FN Thomson Reuters Web of Science™ VR 1.0 PT J AU Smeets, PJM Cho, KR Kempen, RGE Sommerdijk, NAJM De Yoreo, JJ AF Smeets, Paul J. M. Cho, Kang Rae Kempen, Ralph G. E. Sommerdijk, Nico A. J. M. De Yoreo, James J. TI Calcium carbonate nucleation driven by ion binding in a biomimetic matrix revealed by in situ electron microscopy SO NATURE MATERIALS LA English DT Article ID CRYSTAL NUCLEATION; GROWTH; BIOMINERALIZATION; LIQUID; SYSTEMS; TEM; MINERALIZATION; TEMPLATE; ENERGIES; KINETICS AB The characteristic shapes, structures and properties of biominerals arise from their interplay with a macromolecular matrix(1,2). The developing mineral interacts with acidic macromolecules, which are either dissolved in the crystallization medium or associated with insoluble matrix polymers(3), that affect growth habits and phase selection or completely inhibit precipitation in solution(4-6). Yet little is known about the role of matrix-immobilized acidic macromolecules in directing mineralization. Here, by using in situ liquid-phase electron microscopy to visualize the nucleation and growth of CaCO3 in a matrix of polystyrene sulphonate (PSS), we show that the binding of calcium ions to form Ca-PSS globules is a key step in the formation of metastable amorphous calcium carbonate (ACC), an important precursor phase in many biomineralization systems(7). Our findings demonstrate that ion binding can play a significant role in directing nucleation, independently of any control over the free-energy barrier to nucleation. C1 [Smeets, Paul J. M.; Cho, Kang Rae] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Smeets, Paul J. M.; Kempen, Ralph G. E.; Sommerdijk, Nico A. J. M.] Eindhoven Univ Technol, Lab Mat & Interface Chem, NL-5600 MB Eindhoven, Netherlands. [Smeets, Paul J. M.; Kempen, Ralph G. E.; Sommerdijk, Nico A. J. M.] Eindhoven Univ Technol, Soft Matter CryoTEM Unit, NL-5600 MB Eindhoven, Netherlands. [Smeets, Paul J. M.; Sommerdijk, Nico A. J. M.] Eindhoven Univ Technol, Inst Complex Mol Syst, NL-5600 MB Eindhoven, Netherlands. [Smeets, Paul J. M.; De Yoreo, James J.] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. RP Sommerdijk, NAJM (reprint author), Eindhoven Univ Technol, Lab Mat & Interface Chem, POB 513, NL-5600 MB Eindhoven, Netherlands. EM N.Sommerdijk@tue.nl; james.deyoreo@pnnl.gov RI Foundry, Molecular/G-9968-2014; Sommerdijk, Nico/B-7239-2013; OI Sommerdijk, Nico/0000-0002-8956-195X; Smeets, Paul/0000-0002-7281-0120 FU US Department of Energy, Office of Basic Energy Sciences, at Lawrence Berkeley National Laboratory; US Department of Energy [DE-AC05-76RL01830]; VICI grant of the Dutch Science Foundation, NWO, The Netherlands FX We thank V. Altoe and S. Aloni for the use of, and assistance with, the JEOL-2100F, J. Tao for help with confocal Raman microscopy, and H. Friedrich and M. Nielsen for help with TEM data analysis. This research was supported by the US Department of Energy, Office of Basic Energy Sciences, at Lawrence Berkeley National Laboratory and at the Pacific Northwest National Laboratory (PNNL). Characterization of PSS globule formation was supported by the Materials Science and Engineering Division. Investigation of calcium carbonate nucleation was supported by the Division of Chemical Sciences, Geosciences, and Biosciences. Transmission electron microscopy was performed at the Molecular Foundry, Lawrence Berkeley National Laboratory, which is supported by the Office of Basic Energy Sciences, Scientific User Facilities Division. PNNL is operated by Battelle for the US Department of Energy under Contract DE-AC05-76RL01830. The work of P.J.M.S. and N.A.J.M.S. is supported by a VICI grant of the Dutch Science Foundation, NWO, The Netherlands. NR 39 TC 66 Z9 66 U1 53 U2 227 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1476-1122 EI 1476-4660 J9 NAT MATER JI Nat. Mater. PD APR PY 2015 VL 14 IS 4 BP 394 EP 399 DI 10.1038/NMAT4193 PG 6 WC Chemistry, Physical; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Materials Science; Physics GA CE3VN UT WOS:000351757800013 PM 25622001 ER PT J AU Sachet, E Shelton, CT Harris, JS Gaddy, BE Irving, DL Curtarolo, S Donovan, BF Hopkins, PE Sharma, PA Sharma, AL Ihlefeld, J Franzen, S Maria, JP AF Sachet, Edward Shelton, Christopher T. Harris, Joshua S. Gaddy, Benjamin E. Irving, Douglas L. Curtarolo, Stefano Donovan, Brian F. Hopkins, Patrick E. Sharma, Peter A. Sharma, Ana Lima Ihlefeld, Jon Franzen, Stefan Maria, Jon-Paul TI Dysprosium-doped cadmium oxide as a gateway material for mid-infrared plasmonics SO NATURE MATERIALS LA English DT Article ID INITIO MOLECULAR-DYNAMICS; GRAPHENE; METALS; FILMS; CDO AB The interest in plasmonic technologies surrounds many emergent optoelectronic applications, such as plasmon lasers, transistors, sensors and information storage. Although plasmonic materials for ultraviolet-visible and near-infrared wavelengths have been found, the mid-infrared range remains a challenge to address: few known systems can achieve subwavelength optical confinement with low loss in this range. With a combination of experiments and ab initio modelling, here we demonstrate an extreme peak of electron mobility in Dy-doped CdO that is achieved through accurate 'defect equilibrium engineering'. In so doing, we create a tunable plasmon host that satisfies the criteria for mid-infrared spectrum plasmonics, and overcomes the losses seen in conventional plasmonic materials. In particular, extrinsic doping pins the CdO Fermi level above the conduction band minimum and it increases the formation energy of native oxygen vacancies, thus reducing their populations by several orders of magnitude. The substitutional lattice strain induced by Dy doping is sufficiently small, allowing mobility values around 500 cm(2) V-1 s(-1) for carrier densities above 10(20) cm(3). Our work shows that CdO: Dy is a model system for intrinsic and extrinsic manipulation of defects affecting electrical, optical and thermal properties, that oxide conductors are ideal candidates for plasmonic devices and that the defect engineering approach for property optimization is generally applicable to other conducting metal oxides. C1 [Sachet, Edward; Shelton, Christopher T.; Harris, Joshua S.; Gaddy, Benjamin E.; Irving, Douglas L.; Maria, Jon-Paul] N Carolina State Univ, Dept Mat Sci, Raleigh, NC 27695 USA. [Curtarolo, Stefano] Duke Univ, Dept Mech Engn & Mat Sci, Durham, NC 27708 USA. [Curtarolo, Stefano] Duke Univ, Dept Elect Engn, Durham, NC 27708 USA. [Donovan, Brian F.] Univ Virginia, Dept Mat Sci & Engn, Charlottesville, VA 22904 USA. [Hopkins, Patrick E.] Univ Virginia, Dept Mech & Aerosp Engn, Charlottesville, VA 22904 USA. [Sharma, Peter A.; Sharma, Ana Lima; Ihlefeld, Jon] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Franzen, Stefan] N Carolina State Univ, Dept Chem, Raleigh, NC 27695 USA. RP Curtarolo, S (reprint author), Duke Univ, Dept Mech Engn & Mat Sci, Durham, NC 27708 USA. EM stefano.curtarolo@duke.edu; jpmaria@ncsu.edu FU NSF grant [CHE-1112017, DMR-1151568]; US Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; Air Force Office of Scientific Research under AFOSR [FA9550-14-1-0067, 5010-UV-AFOSR-0067]; ONR Young Investigator Program [N00014-13-4-0528]; Duke Center for Materials Genomics; ONR [MURI N00014-13-1-0635] FX S.F. and J-P.M. gratefully acknowledge support of this work by NSF grant CHE-1112017. The NSF grant DMR-1151568 supported the DFT contributions. We would further like to acknowledge Efimenko and Genzer (NCSU, CBE) for granting us access to the IR-Ellipsometer. Sandia National Laboratories is a multi-programme laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the US Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. The thermal conductivity measurements were supported by the Air Force Office of Scientific Research under AFOSR Award No. FA9550-14-1-0067 (Subaward No. 5010-UV-AFOSR-0067) and the ONR Young Investigator Program (N00014-13-4-0528). S.C. acknowledges the Duke Center for Materials Genomics and partial support by ONR (MURI N00014-13-1-0635). NR 38 TC 25 Z9 25 U1 16 U2 113 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1476-1122 EI 1476-4660 J9 NAT MATER JI Nat. Mater. PD APR PY 2015 VL 14 IS 4 BP 414 EP 420 DI 10.1038/NMAT4203 PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Materials Science; Physics GA CE3VN UT WOS:000351757800016 PM 25686264 ER PT J AU Busby, E Xia, JL Wu, Q Low, JZ Song, R Miller, JR Zhu, XY Campos, LM Sfeir, MY AF Busby, Erik Xia, Jianlong Wu, Qin Low, Jonathan Z. Song, Rui Miller, John R. Zhu, X-Y. Campos, Luis M. Sfeir, Matthew Y. TI A design strategy for intramolecular singlet fission mediated by charge-transfer states in donor-acceptor organic materials SO NATURE MATERIALS LA English DT Article ID TIME-RESOLVED SPECTRA; SOLAR-CELLS; BAND-GAP; CONJUGATED POLYMERS; OPTICAL-PROPERTIES; ENERGY-TRANSFER; CONVERSION; CAROTENOIDS; RELAXATION; EFFICIENCY AB The ability to advance our understanding of multiple exciton generation (MEG) in organic materials has been restricted by the limited number of materials capable of singlet fission. A particular challenge is the development of materials that undergo efficient intramolecular fission, such that local order and strong nearest-neighbour coupling is no longer a design constraint. Here we address these challenges by demonstrating that strong intrachain donor-acceptor interactions are a key design feature for organic materials capable of intramolecular singlet fission. By conjugating strong-acceptor and strong-donor building blocks, small molecules and polymers with charge-transfer states that mediate population transfer between singlet excitons and triplet excitons are synthesized. Using transient optical techniques, we show that triplet populations can be generated with yields up to 170%. These guidelines are widely applicable to similar families of polymers and small molecules, and can lead to the development of new fission-capable materials with tunable electronic structure, as well as a deeper fundamental understanding of MEG. C1 [Busby, Erik; Xia, Jianlong; Zhu, X-Y.; Campos, Luis M.] Columbia Univ, Energy Frontier Res Ctr, New York, NY 10027 USA. [Busby, Erik; Wu, Qin; Sfeir, Matthew Y.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Xia, Jianlong; Low, Jonathan Z.; Song, Rui; Zhu, X-Y.; Campos, Luis M.] Columbia Univ, Dept Chem, New York, NY 10027 USA. [Miller, John R.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. RP Campos, LM (reprint author), Columbia Univ, Energy Frontier Res Ctr, New York, NY 10027 USA. EM lcampos@columbia.edu; msfeir@bnl.gov RI Xia, Jianlong/I-9076-2012; Wu, Qin/C-9483-2009; OI Wu, Qin/0000-0001-6350-6672; Sfeir, Matthew/0000-0001-5619-5722 FU Center for Re-Defining Photovoltaic Efficiency Through Molecular-Scale Control, an Energy Frontier Research Center - US Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences [DE-SC0001085]; 3M Non-Tenured Faculty Award; NSF CAREER [DMR-1351293]; National Science Foundation [DMR-1321405]; US Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886]; Chemistry Department, Brookhaven National Laboratory [DE-AC02-98-CH10886] FX This project was funded through the Center for Re-Defining Photovoltaic Efficiency Through Molecular-Scale Control, an Energy Frontier Research Center funded by the US Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences under Award DE-SC0001085. L.M.C. thanks 3M Non-Tenured Faculty Award and the NSF CAREER (DMR-1351293) for funding the synthesis of the small molecules and control materials. X-Y.Z. acknowledges support by the National Science Foundation, DMR-1321405. We wish to thank M. Vengris (Vilnius University) for graciously providing his global analysis software package for our use. We also thank S. Wei for a sample of PFTDO1 and J. Hoy for additional cyclic voltammetry measurements. Research was carried out in part at the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the US Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886, and in the Chemistry Department, Brookhaven National Laboratory through Grant #DE-AC02-98-CH10886, which also supports the LEAF Facility of the BNL Accelerator Center for Energy Research. NR 47 TC 56 Z9 56 U1 28 U2 194 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1476-1122 EI 1476-4660 J9 NAT MATER JI Nat. Mater. PD APR PY 2015 VL 14 IS 4 BP 426 EP 433 DI 10.1038/NMAT4175 PG 8 WC Chemistry, Physical; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Materials Science; Physics GA CE3VN UT WOS:000351757800018 PM 25581625 ER PT J AU Dickman, LT McDowell, NG Sevanto, S Pangle, RE Pockman, WT AF Dickman, Lee T. McDowell, Nate G. Sevanto, Sanna Pangle, Robert E. Pockman, William T. TI Carbohydrate dynamics and mortality in a pinon-juniper woodland under three future precipitation scenarios SO PLANT CELL AND ENVIRONMENT LA English DT Article DE anisohydric; climate; die-off; hydraulics; isohydric; plant; storage; sugars; vegetation; water relations ID INDUCED TREE MORTALITY; PLANT HYDRAULIC CONDUCTANCE; DROUGHT-INDUCED MORTALITY; LEAF GAS-EXCHANGE; SOLUTE ACCUMULATION; OSMOTIC ADJUSTMENT; CLIMATE-CHANGE; WATER-STRESS; VEGETATION MORTALITY; CARBON METABOLISM AB Drought-induced forest mortality is an increasing global problem with wide-ranging consequences, yet mortality mechanisms remain poorly understood. Depletion of non-structural carbohydrate (NSC) stores has been implicated as an important mechanism in drought-induced mortality, but experimental field tests are rare. We used an ecosystem-scale precipitation manipulation experiment to evaluate leaf and twig NSC dynamics of two co-occurring conifers that differ in patterns of stomatal regulation of water loss and recent mortality: the relatively desiccation-avoiding pinon pine (Pinus edulis) and the relatively desiccation-tolerant one-seed juniper (Juniperus monosperma). Pinon pine experienced 72% mortality after 13-25 months of experimental drought and juniper experienced 20% mortality after 32-47 months. Juniper maintained three times more NSC in the foliage than twigs, and converted NSC to glucose and fructose under drought, consistent with osmoregulation requirements to maintain higher stomatal conductance during drought than pinon. Despite these species differences, experimental drought caused decreased leaf starch content in dying trees of both species (P<0.001). Average dry-season leaf starch content was also a good predictor of drought-survival time for both species (R-2=0.93). These results, along with observations of drought-induced reductions to photosynthesis and growth, support carbon limitation as an important process during mortality of these two conifer species. C1 [Dickman, Lee T.; McDowell, Nate G.; Sevanto, Sanna] Los Alamos Natl Lab, Div Earth & Environm Sci, Los Alamos, NM 87545 USA. [Pangle, Robert E.; Pockman, William T.] Univ New Mexico, Dept Biol, Albuquerque, NM 87131 USA. RP Dickman, LT (reprint author), Los Alamos Natl Lab, Div Earth & Environm Sci, Los Alamos, NM 87545 USA. EM lee@lanl.gov RI Dickman, Lee/J-2391-2015; Pockman, William/D-4086-2014 OI Dickman, Lee/0000-0003-3876-7058; Pockman, William/0000-0002-3286-0457 FU Department of Energy's Office of Science (BER); Sevilleta LTER program [NSF DEB-0620482]; UNM Sevilleta Field Station FX Many thanks to Judson Hill, Enrico Yepez, David Fox, Clif Meyer and countless undergraduate assistants for helping to implement this experiment and carry out numerous field campaigns and NSC analyses. We are also indebted to Dr Larry Ticknor, Dr Tom Burr, and Dr Park Williams for their guidance with statistical analysis. This project was funded by the Department of Energy's Office of Science (BER) with additional support from the Sevilleta LTER program (NSF DEB-0620482) and UNM Sevilleta Field Station. NR 64 TC 16 Z9 16 U1 8 U2 78 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0140-7791 EI 1365-3040 J9 PLANT CELL ENVIRON JI Plant Cell Environ. PD APR PY 2015 VL 38 IS 4 BP 729 EP 739 DI 10.1111/pce.12441 PG 11 WC Plant Sciences SC Plant Sciences GA CD8XC UT WOS:000351378800010 PM 25159277 ER PT J AU Wei, STS Fernandez-Martinez, MA Chan, YK Van Nostrand, JD de los Rios-Murillo, A Chiu, JMY Ganeshram, AM Cary, SC Zhou, JZ Pointing, SB AF Wei, Sean T. S. Fernandez-Martinez, Miguel-Angel Chan, Yuki Van Nostrand, Joy D. de los Rios-Murillo, Asuncion Chiu, Jill M. Y. Ganeshram, Annapoorna Maitrayee Cary, S. Craig Zhou, Jizhong Pointing, Stephen B. TI Diverse metabolic and stress-tolerance pathways in chasmoendolithic and soil communities of Miers Valley, McMurdo Dry Valleys, Antarctica SO POLAR BIOLOGY LA English DT Article DE Antarctica; Chasmoendolith; Dry Valleys; Geochip; Stress response ID HYPOLITHIC MICROBIAL COMMUNITIES; COLD DESERTS; CYANOBACTERIA; NITROGEN; HOT; MICROSCOPY; GRANITE; ECOLOGY; CYCLES; ROCKS AB The majority of biomass in the McMurdo Dry Valleys of Antarctica occurs within rocks and soils, but despite the wealth of biodiversity data very little is known about the potential functionality of communities within these substrates. The putative physiological capacity of microbial communities in granite boulders (chasmoendoliths) and soils of a maritime-influenced Antarctic Dry Valleys were interrogated using the GeoChip microarray. Diversity estimates revealed surprisingly high diversity and evenness in both communities, with Chlorobi and Deinococci in soils accounting for major differences between the substrates. Autotrophs were more diverse in chasmoendoliths, and diazotrophs more diverse in soils. Both substrates revealed a previously unappreciated abundance of Halobacteria (Archaea), Ascomycota (Fungi) and Basidiomycoyta (Fungi). The fungi accounted for much of the differences between substrates in metabolic pathways associated with carbon transformations, particularly for aromatic compounds. Nitrogen fixation genes were more common in soils, although nitrogen catabolism genes were abundant in chasmoendoliths. Stress response pathways were more diverse in chasmoendoliths, possibly reflecting greater environmental stress in this exposed substrate compared with subsurface soils. Overall diversity of stress-tolerance genes was markedly lower than that recorded for inland locations where environmental stress is exacerbated. We postulate that the chasmoendolithic community occupies a key role in biogeochemical transformations in Dry Valley systems where granite substrates are abundant among open soils. The findings indicate that a substantial upward revision to estimates of biologically active surfaces in this system is warranted. C1 [Wei, Sean T. S.; Chan, Yuki; Ganeshram, Annapoorna Maitrayee; Pointing, Stephen B.] Auckland Univ Technol, Inst Appl Ecol New Zealand, Sch Appl Sci, Auckland 1142, New Zealand. [Fernandez-Martinez, Miguel-Angel; de los Rios-Murillo, Asuncion] Ctr Ciencias Medioambientales, Madrid 28006, Spain. [Van Nostrand, Joy D.; Zhou, Jizhong] Univ Oklahoma, Inst Environm Genom, Dept Microbiol & Plant Biol, Norman, OK 73019 USA. [Chiu, Jill M. Y.] Hong Kong Baptist Univ, Dept Biol, Kowloon Tong, Hong Kong, Peoples R China. [Cary, S. Craig; Pointing, Stephen B.] Univ Waikato, Int Ctr Terr Antarctic Res, Hamilton 3240, New Zealand. [Zhou, Jizhong] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Zhou, Jizhong] Tsinghua Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100084, Peoples R China. RP Pointing, SB (reprint author), Auckland Univ Technol, Inst Appl Ecol New Zealand, Sch Appl Sci, Private Bag 92006, Auckland 1142, New Zealand. EM steve.pointing@aut.ac.nz RI de los Rios, Asuncion/L-3694-2014; Van Nostrand, Joy/F-1740-2016; Wei, Sean/A-5878-2017; OI de los Rios, Asuncion/0000-0002-0266-3516; Van Nostrand, Joy/0000-0001-9548-6450; Wei, Sean/0000-0003-3783-6429; Chan, Yuki/0000-0002-9570-5462 FU Institute for Applied Ecology New Zealand; Ecosystems and Networks Integrated with Genes and Molecular Assemblies (ENIGMA) through the US Department of Energy [DE-AC02-05CH11231]; US Department of Energy [DE-SC0004601]; US National Science Foundation [EF-1065844] FX This study was funded by the Institute for Applied Ecology New Zealand. The development of the GeoChip and associated computational pipelines used in this study was supported by Ecosystems and Networks Integrated with Genes and Molecular Assemblies (ENIGMA) through the US Department of Energy (DE-AC02-05CH11231). J. Zhou and J. D. Van Nostrand's efforts were supported by the US Department of Energy (DE-SC0004601) and the US National Science Foundation (EF-1065844). The authors are extremely grateful to Antarctica New Zealand for logistics and field support in Antarctica. NR 38 TC 1 Z9 1 U1 3 U2 21 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0722-4060 EI 1432-2056 J9 POLAR BIOL JI Polar Biol. PD APR PY 2015 VL 38 IS 4 BP 433 EP 443 DI 10.1007/s00300-014-1598-3 PG 11 WC Biodiversity Conservation; Ecology SC Biodiversity & Conservation; Environmental Sciences & Ecology GA CD6DG UT WOS:000351179000001 ER PT J AU Busch, AWU Montgomery, BL AF Busch, Andrea W. U. Montgomery, Beronda L. TI Interdependence of tetrapyrrole metabolism, the generation of oxidative stress and the mitigative oxidative stress response SO REDOX BIOLOGY LA English DT Review DE High light; Iron; Oxidative stress; Photosynthesis; ROS; Tetrapyrrole ID PERIPHERAL BENZODIAZEPINE-RECEPTOR; THIOL/DISULFIDE REDOX SWITCH; MG-PROTOPORPHYRIN IX; SP PCC 7120; MITOCHONDRIAL PERMEABILITY TRANSITION; CYANOBACTERIUM FREMYELLA-DIPLOSIPHON; PHYTOCHROME-INTERACTING FACTORS; LIGHT-DEPENDENT REGULATION; SINGLET OXYGEN PRODUCTION; SYNECHOCOCCUS SP PCC7942 AB Tetrapyrroles are involved in light harvesting and light perception, electron transfer reactions, and as cofactors for key enzymes and sensory proteins. Under conditions in which cells exhibit stress-induced imbalances of photosynthetic reactions, or light absorption exceeds the ability of the cell to use photoexcitation energy in synthesis reactions, redox imbalance can occur in photosynthetic cells. Such conditions can lead to the generation of reactive oxygen species (ROS) associated with alterations in tetrapyrrole homeostasis. ROS accumulation can result in cellular damage and detrimental effects on organismal Fitness, or ROS molecules can serve as signals to induce a protective or damage-mitigating oxidative stress signaling response in cells. Induced oxidative stress responses include tetrapyrrole-dependent and -independent mechanisms for mitigating ROS generation and/or accumulation. Thus, tetrapyrroles can be contributors to oxidative stress, but are also essential in the oxidative stress response to protect cells by contributing to detoxification of ROS. In this review, we highlight the interconnection and interdependence of tetrapyrrole metabolism with the occurrence of oxidative stress and protective oxidative stress signaling responses in photosynthetic organisms. (C) 2015 The Authprs. Published by Elsevier By. C1 [Busch, Andrea W. U.; Montgomery, Beronda L.] Michigan State Univ, Plant Res Lab, Dept Energy, E Lansing, MI 48824 USA. [Montgomery, Beronda L.] Michigan State Univ, Dept Biochem & Mol Biol, E Lansing, MI 48824 USA. RP Montgomery, BL (reprint author), Michigan State Univ, Plant Res Lab, US DOE, 612 Wilson Rd, E Lansing, MI 48824 USA. EM montg133@msu.edu FU National Science Foundation [MCB-1243983]; U.S. Department of Energy (Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Sciences, Office of Science) [DE-FG] FX Work in the corresponding author's laboratory is funded by the National Science Foundation for investigations into light signaling and adaptation in cyanobacteria (No. MCB-1243983 to BLM) and by the U.S. Department of Energy (Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Sciences, Office of Science, Grant no. DE-FG to BLM). We would like to thank Marlene Cameron for assistance with graphic design. NR 178 TC 11 Z9 11 U1 5 U2 23 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 2213-2317 J9 REDOX BIOL JI Redox Biol. PD APR PY 2015 VL 4 BP 260 EP 271 DI 10.1016/j.redox.2015.01.010 PG 12 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CD1DI UT WOS:000350813800029 PM 25618582 ER PT J AU Hacene, MAB Sari, NEC Benzair, A Berkovitz, R AF Hacene, M. A. Boukli Sari, N. E. Chabane Benzair, A. Berkovitz, R. TI Application of a sustainable energy system for house energy needs in Tlemcen (North Africa) SO RENEWABLE & SUSTAINABLE ENERGY REVIEWS LA English DT Review DE Heat pump; Diffusivity; Collector; Depth; Temperature AB This article highlights a method for natural heating and cooling of systems in areas of moderate climate. Movement of air is generated in the system by an underground piping system. In this paper, we discuss a feasibility study in Algeria of air-conditioning using a ground source heat pump (GSHP) with vertical mounting, coupled with a solar collector. This study consists of modeling ground temperature at different depths, for a clay soil in the city of Tlemcen. Our model is developed from the non-stationary heat equation for a homogeneous medium and takes into consideration the soil thermal diffusivity. It uses the daily ambient temperature during a typical year for the locality of Tlemcen. The study shows the feasibility of using a heating/cooling GSHP in the town of Tlemcen for the particular soil type, and indicates that the duration of air flow in the borehole has a major influence on the outgoing temperature drilling. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Hacene, M. A. Boukli; Sari, N. E. Chabane] Abou Baker Belkaid Univ, Mat & Renewable Energy Res Unit URMER, Tilimsen 13000, Algeria. [Hacene, M. A. Boukli; Benzair, A.] Djillali Liabes Univ Sidi Bel Abbes, Sidi Bel Abbes 22000, Algeria. [Berkovitz, R.] Univ Calif, Lawrence Berkeley Natl Labs, Berkeley, CA USA. RP Hacene, MAB (reprint author), Abou Baker Belkaid Univ, Mat & Renewable Energy Res Unit URMER, PB 119, Tilimsen 13000, Algeria. EM amineboukli@yahoo.fr NR 20 TC 2 Z9 2 U1 2 U2 11 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1364-0321 J9 RENEW SUST ENERG REV JI Renew. Sust. Energ. Rev. PD APR PY 2015 VL 44 BP 109 EP 116 DI 10.1016/j.rser.2014.12.007 PG 8 WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Energy & Fuels SC Science & Technology - Other Topics; Energy & Fuels GA CD8DB UT WOS:000351324300010 ER PT J AU Jia, Y Sun, CH Shen, SH Zou, J Mao, SS Yao, XD AF Jia, Yi Sun, Chenghua Shen, Shaohua Zou, Jin Mao, Samuel S. Yao, Xiangdong TI Combination of nanosizing and interfacial effect: Future perspective for designing Mg-based nanomaterials for hydrogen storage SO RENEWABLE & SUSTAINABLE ENERGY REVIEWS LA English DT Review DE Mg based hydrogen storage materials; Size effect; Interface effect; Thermodynamics; Kinetics ID METAL-ORGANIC FRAMEWORKS; BALL-MILLED MGH2; MAGNESIUM HYDRIDE; SORPTION PROPERTIES; HIGH-CAPACITY; MELT INFILTRATION; ENERGY-PRODUCTION; CARBON NANOTUBES; COMPLEX HYDRIDES; GRAPHITE CARBON AB Hydrogen storage is now the "bottle neck" to realize application of hydrogen as the renewable energy. The breakthrough in hydrogen storage is quite urgent. Magnesium is a promising candidate for hydrogen storage that attracts tremendous interest in last a few decades and significant progress has been made in recent years. Accordingly, in this article, we comprehensively reviewed different strategies to overcome the key barriers of high desorption temperature and low kinetics, especially on the recent approaches of nanosizing and interfacial confinement. We also try to give our own point of view on the future perspectives of research in Mg for hydrogen storage. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Jia, Yi; Yao, Xiangdong] Griffith Univ, Sch Nat Sci, Brisbane, Qld 4111, Australia. [Jia, Yi; Zou, Jin] Univ Queensland, Sch Mech & Min Engn, Brisbane, Qld 4072, Australia. [Sun, Chenghua] Univ Queensland, Ctr Computat Mol Sci, Brisbane, Qld 4072, Australia. [Shen, Shaohua] Xi An Jiao Tong Univ, Int Res Ctr Renewable Energy, State Key Lab Multiphase Flow Power Engn, Xian 710049, Shaanxi, Peoples R China. [Shen, Shaohua; Mao, Samuel S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Mech Engn, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Zou, Jin] Univ Queensland, CMM, Brisbane, Qld 4072, Australia. [Yao, Xiangdong] Griffith Univ, QMNC, Brisbane, Qld 4111, Australia. [Sun, Chenghua] Monash Univ, Fac Sci, Sch Chem, Clayton, Vic 3800, Australia. RP Mao, SS (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Mech Engn, Environm Energy Technol Div, Berkeley, CA 94720 USA. EM SSMao@lbl.gov; x.yao@griffith.edu.au RI Zou, Jin/B-3183-2009; Yao, Xiangdong/E-1259-2013; Griffith University, QMNC/I-5498-2013; Shen, Shaohua/E-9507-2011 OI Zou, Jin/0000-0001-9435-8043; FU Australia Research Council [DP0986382]; University of Queensland FX The financial support from Australia Research Council (DP0986382) is appreciated. Dr. Yi Jia also thanks the University of Queensland's travel award to support his collaborative research at UC Berkeley. NR 142 TC 25 Z9 26 U1 25 U2 167 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1364-0321 J9 RENEW SUST ENERG REV JI Renew. Sust. Energ. Rev. PD APR PY 2015 VL 44 BP 289 EP 303 DI 10.1016/j.rser.2014.12.032 PG 15 WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Energy & Fuels SC Science & Technology - Other Topics; Energy & Fuels GA CD8DB UT WOS:000351324300021 ER PT J AU Yang, XF Haas, KA Fritz, HM French, SP Shi, X Neary, VS Gunawan, B AF Yang, Xiufeng Haas, Kevin A. Fritz, Hermann M. French, Steven P. Shi, Xuan Neary, Vincent S. Gunawan, Budi TI National geodatabase of ocean current power resource in USA SO RENEWABLE & SUSTAINABLE ENERGY REVIEWS LA English DT Review DE Ocean currents; Hydrokinetic energy; Gulf Stream system; Resource assessment ID GULF-STREAM; FLORIDA CURRENT; VERTICAL COORDINATE; ENERGY; VARIABILITY; CIRCULATION; TRANSPORT AB Ocean currents represent an alternative source of clean energy given their inherent reliability, persistence and sustainability. The general ocean circulation is characterized by large rotating ocean gyres resulting in rapid ocean currents along the western boundaries because of the Coriolis Effect. The Gulf Stream system is formed by the western boundary current of the North Atlantic Ocean flowing along the east coast of the United States, and is of particular interest as a potential energy resource for the United States. This study presents a national database of ocean current kinetic energy resource derived from seven years of numerical model simulations to help advance awareness and market penetration for ocean current energy. A web based GIS interface is provided for dissemination of the national energy resource data: http://www.oceancurrentpower.gatech.edu/. The website includes GIS layers of computed monthly and yearly mean ocean current speed and associated power density along the coastlines of the United States, as well as joint and marginal probability histograms for current velocities at a variable horizontal resolution of 4-7 km. Various tools are provided for viewing, identifying, filtering and downloading the data from this website. The Gulf Stream system, especially the Florida Current, concentrates the highest kinetic power density (> 2000 W/m(2)). The majority of the kinetic power and its variability are only present in relatively shallow water given the strong correlation with the surface wind stress. The kinetic energy flux in the Florida Current is estimated over 30 years to provide temporal variability of the undisturbed kinetic energy with high statistical significance. Available power of approximately 5 GW associated with the undisturbed natural flow condition from the Gulf Stream system is predicted based on hypothetical turbine parameters. Successful development of renewable energy generation requires further studies to account for more precise technical, economic and environmental constraints. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Yang, Xiufeng; Haas, Kevin A.; Fritz, Hermann M.] Georgia Inst Technol, Sch Civil & Environm Engn, Atlanta, GA 30332 USA. [French, Steven P.] Georgia Inst Technol, Ctr Geog Informat Syst, Atlanta, GA 30332 USA. [Shi, Xuan] Univ Arkansas, Dept Geosci, Fayetteville, AR 72701 USA. [Neary, Vincent S.; Gunawan, Budi] Sandia Natl Labs, Wind & Water Power Technol, Albuquerque, NM 87185 USA. RP Yang, XF (reprint author), Georgia Inst Technol, Sch Civil & Environm Engn, Atlanta, GA 30332 USA. EM xfyang@gatech.edu RI Fritz, Hermann/H-5618-2013 OI Fritz, Hermann/0000-0002-6798-5401 FU U.S. Department of Energy, Wind and Hydropower Technologies Program [DE-EE0002661] FX This study was supported by the U.S. Department of Energy, Wind and Hydropower Technologies Program award number DE-EE0002661. Any opinions, finding, and conclusions or recommendations expressed herein are those of the authors and do not necessarily reflect the views of the Department of Energy. The authors also want to sincerely thank the HYCOM consortium for sharing HYCOM data. The authors also thank Charlie Barron and Lucy Smedstad from the Naval Research Laboratory for sharing NCOM data. NR 29 TC 3 Z9 3 U1 6 U2 27 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1364-0321 J9 RENEW SUST ENERG REV JI Renew. Sust. Energ. Rev. PD APR PY 2015 VL 44 BP 496 EP 507 DI 10.1016/j.rser.2015.01.007 PG 12 WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Energy & Fuels SC Science & Technology - Other Topics; Energy & Fuels GA CD8DB UT WOS:000351324300035 ER PT J AU Shilling, R AF Shilling, Russell TI The Case for Education Moon Shots SO SCIENTIFIC AMERICAN LA English DT Editorial Material C1 [Shilling, Russell] US DOE, STEM, Washington, DC 20585 USA. RP Shilling, R (reprint author), US DOE, STEM, Washington, DC 20585 USA. NR 0 TC 0 Z9 0 U1 0 U2 2 PU NATURE PUBLISHING GROUP PI NEW YORK PA 75 VARICK ST, 9TH FLR, NEW YORK, NY 10013-1917 USA SN 0036-8733 J9 SCI AM JI Sci.Am. PD APR PY 2015 VL 312 IS 4 BP 12 EP 12 PG 1 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CD6IO UT WOS:000351193000011 ER PT J AU Liu, YW Ouyang, XP Durakiewicz, T Halas, S Wang, XF AF Liu, Y. W. Ouyang, X. P. Durakiewicz, T. Halas, S. Wang, X. F. TI Impact of nitrogen on effective work function of metal/oxide stack: A first-principles study of the Pt/HfO2 interface SO SOLID STATE COMMUNICATIONS LA English DT Article DE Metal/oxide interface; N dopant; Work function; First-principles study ID ELECTRONIC-STRUCTURE; METAL; TECHNOLOGY AB Modulating the effective work function (Phi(eff)) of metal electrodes is both crucial and challenging in metal-oxide-semiconductor transistors. The introduction of atomic dopants is shown to be an effective method to modify the interface Phi(eff). Here we apply the first principles calculations to systematically explore the impact of incorporation of the non-metallic ambient gas element N On the effective work Function of a Pt/HfO2 interface. We find that Phi(eff) is very closely related to the doped atomic position and concentration of the incorporated N atoms. The incorporation is favored at the interface near HfO2 side. and it can significantly increase the interface Phi(eff) for the Pt/HfO2 stack (making it more p-type). Also, the Phi(eff) increases with the increase of doped N concentration clue to the mitigation effect of doped N on interface dipole moment. Our findings will provide guidance in developing the environment annealing approach to modulation of Phi(eff) of the metal/oxide stack. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Liu, Y. W.; Ouyang, X. P.; Wang, X. F.] Xiangtan Univ, Sch Mat Sci & Engn, Xiangtan 411105, Hunan, Peoples R China. [Ouyang, X. P.] Northwest Inst Nucl Technol, Xian 710024, Shanxi, Peoples R China. [Durakiewicz, T.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Halas, S.] Marie Curie Sklodowska Univ, Inst Phys, PL-20031 Lublin, Poland. RP Wang, XF (reprint author), Xiangtan Univ, Sch Mat Sci & Engn, Xiangtan 411105, Hunan, Peoples R China. EM onexf@xtu.edu.cn FU National Natural Science Foundation of China [11202178, 11275150, 11435010]; Natural Science Foundation of Hunan Province [14JJ3082]; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division FX We gratefully acknowledge support of this work by the National Natural Science Foundation of China (11202178, 11275150, 11435010) and Natural Science Foundation of Hunan Province (14JJ3082), Works at LANL was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. NR 22 TC 0 Z9 0 U1 2 U2 18 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0038-1098 EI 1879-2766 J9 SOLID STATE COMMUN JI Solid State Commun. PD APR PY 2015 VL 207 BP 44 EP 48 DI 10.1010/j.ssc.2015.01.017 PG 5 WC Physics, Condensed Matter SC Physics GA CD8JK UT WOS:000351340900010 ER PT J AU Gautam, A Ophus, C Lancon, F Denes, P Dahmen, U AF Gautam, A. Ophus, C. Lancon, F. Denes, P. Dahmen, U. TI Analysis of grain boundary dynamics using event detection and cumulative averaging SO ULTRAMICROSCOPY LA English DT Article; Proceedings Paper CT PICO 2015: 3rd Conference on Frontiers of Aberration Corrected Electron Microscopy CY APR 19-23, 2015 CL Vaals, NETHERLANDS DE HRTEM; HAADF; Dynamics; Atomic structure; Grain boundaiy; Simulation; Step; Time average; Aberration correction; Electron detector ID ACTIVE PIXEL SENSOR; ELECTRON-MICROSCOPY; ATOMIC-STRUCTURE; MOTION; INTERFACE; MECHANISM; MIGRATION; MODEL; FILMS; GOLD AB To analyze exlended Lime series of high resolulion images, we have employed automated frame-by-frame comparisons that are able to detect dynamic changes in the structure of a grain boundary in Au. Using cumulative averaging of images between events allowed high resolution measurements of the atomic relaxation in the interface with sufficient accuracy for comparison with atomistic models. Cumulative averaging was also used to observe the structural rearrangement of atomic columns at a moving step in the grain boundary. The technique of analyzing changing features in high resolution images by averaging between incidents can be used to deconvolute stochastic events that occur at random intervals and on time scales well beyond that accessible to single-shot imaging. (C) 2014 Elsevier B.V. All rights reserved. C1 [Gautam, A.; Ophus, C.; Denes, P.; Dahmen, U.] Natl Ctr Electron Microscopy, LBNL, Berkeley, CA 94720 USA. [Lancon, F.] CEA Grenoble, INAC, SP2M, Lab Simulat Atomist L Sim, F-38054 Grenoble, France. RP Dahmen, U (reprint author), Natl Ctr Electron Microscopy, LBNL, Berkeley, CA 94720 USA. EM udahmen@lbl.gov RI Foundry, Molecular/G-9968-2014; OI Ophus, Colin/0000-0003-2348-8558 FU Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-ACO3-765FOOO98]; Direction des Sciences de la Matiere of the CEA FX This work is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-ACO3-765FOOO98, and by the Direction des Sciences de la Matiere of the CEA. NR 30 TC 1 Z9 1 U1 1 U2 10 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0304-3991 EI 1879-2723 J9 ULTRAMICROSCOPY JI Ultramicroscopy PD APR PY 2015 VL 151 BP 78 EP 84 DI 10.1016/j.ultramic.2014.11.008 PG 7 WC Microscopy SC Microscopy GA CD6YU UT WOS:000351237800011 PM 25498139 ER PT J AU Ishikawa, R Lupini, AR Hinuma, Y Pennycook, SJ AF Ishikawa, Ryo Lupini, Andrew R. Hinuma, Yoyo Pennycook, Stephen J. TI Large-angle illumination STEM: Toward three-dimensional atom-by-atom imaging SO ULTRAMICROSCOPY LA English DT Article; Proceedings Paper CT PICO 2015: 3rd Conference on Frontiers of Aberration Corrected Electron Microscopy CY APR 19-23, 2015 CL Vaals, NETHERLANDS DE Scanning transmission electron microscopy (STEM); Annular dark-field (ADF); Atomic-depth resolution imaging; Surface imaging ID TRANSMISSION ELECTRON-MICROSCOPY; AUGMENTED-WAVE METHOD; ABERRATION; FIELD; CORRECTORS; SCATTERING; SURFACES; PROBE; TEM AB To fully understand and control materials and their properties, it is of critical importance to determine their atomic structures in all three dimensions. Recent revolutionary advances in electron optics - the inventions of geometric and chromatic aberration correctors as well as electron source monochromators - have provided fertile ground for performing optical depth sectioning at atomic-scale dimensions. In this study we theoretically demonstrate the imaging of top/sub-surface atomic structures and identify the depth of single clopants, single vacancies and the other point defects within materials by large-angle illumination scanning transmission electron microscopy (LAl-STEM). The proposed method also allows us to measure specimen properties such as thickness or three-dimensional surface morphology using observations from a single crystallographic orientation. (C) 2014 Elsevier B.V. All rights reserved. C1 [Ishikawa, Ryo] Univ Tokyo, Inst Engn Innovat, Tokyo 1138656, Japan. [Lupini, Andrew R.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Hinuma, Yoyo] Kyoto Univ, Dept Mat Sci & Engn, Kyoto 6068501, Japan. [Pennycook, Stephen J.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. RP Ishikawa, R (reprint author), Univ Tokyo, Inst Engn Innovat, Tokyo 1138656, Japan. EM ishikawa@sigma.t.u-tokyo.ac.jp OI Ishikawa, Ryo/0000-0001-5801-0971 FU Office of Science of the U.S. DOE [DE-AC02- 05CH11231]; Materials Science and Engineering Division of the US Department of Energy FX RA, acknowledges Prof. Fumiyasu Oba (Kyoto University), Dr. Nathan Lugg, Prof. Naoya Shibata and Prof. Yuichi Ikuhara (University of Tokyo) for helpful discussion careful reading of this manuscript. R.I. and Y.H. support by a Grant-in-Aid for Scientific Research on Innovative Areas "Nano Informatics". RA. used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. DOE under Contract no. DE-AC02- 05CH11231. A.R.L. is supported by the Materials Science and Engineering Division of the US Department of Energy. NR 51 TC 6 Z9 6 U1 2 U2 26 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0304-3991 EI 1879-2723 J9 ULTRAMICROSCOPY JI Ultramicroscopy PD APR PY 2015 VL 151 BP 122 EP 129 DI 10.1016/j.ultramic.2014.11.009 PG 8 WC Microscopy SC Microscopy GA CD6YU UT WOS:000351237800017 PM 25484363 ER PT J AU Pennycook, TJ Lupini, AR Yang, H Murfitt, MF Jones, L Nellist, PD AF Pennycook, Timothy J. Lupini, Andrew R. Yang, Hao Murfitt, Matthew F. Jones, Lewys Nellist, Peter D. TI Efficient phase contrast imaging in STEM using a pixelated detector. Part 1: Experimental demonstration at atomic resolution SO ULTRAMICROSCOPY LA English DT Article; Proceedings Paper CT PICO 2015: 3rd Conference on Frontiers of Aberration Corrected Electron Microscopy CY APR 19-23, 2015 CL Vaals, NETHERLANDS DE STEM; Pixelated detectors; Ptycography; Phase contrast; Chromatic aberrations; DPC; ABF ID TRANSMISSION ELECTRON-MICROSCOPY; INFORMATION LIMIT; PTYCHOGRAPHY AB We demonstrate a method to achieve high efficiency phase contrast imaging in aberration corrected scanning transmission electron microscopy (STEM) with a pixelated detector. The pixelated detector is used to record the Ronchigram as a function of probe position which is then analyzed with ptychography. Ptychography has previously been used to provide super-resolution beyond the diffraction limit of the optics, alongside numerically correcting for spherical aberration. Here we rely on a hardware aberration corrector to eliminate aberrations, but use the pixelated detector data set to utilize the largest possible volume of Fourier space to create high efficiency phase contrast images. The use of ptychography to diagnose the effects of chromatic aberration is also demonstrated. Finally, the four dimensional dataset is used to compare different bright field detector configurations from the same scan for a sample of bilayer graphene. Our method of high efficiency ptychography produces the clearest images, while annular bright field produces almost no contrast for an in-focus aberration-corrected probe. (C) 2014 Elsevier B.V. All rights reserved C1 [Pennycook, Timothy J.; Nellist, Peter D.] SERC, Daresbury Lab, EPSRC SuperSTEM Facil, Warrington WA4 4AD, Cheshire, England. [Pennycook, Timothy J.; Yang, Hao; Jones, Lewys; Nellist, Peter D.] Univ Oxford, Dept Mat, Oxford OX1 3PH, England. [Lupini, Andrew R.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37830 USA. [Murfitt, Matthew F.] Nion Co, Kirkland, WA 98033 USA. RP Pennycook, TJ (reprint author), SERC, Daresbury Lab, EPSRC SuperSTEM Facil, Warrington WA4 4AD, Cheshire, England. EM tpennycook@gmail.com RI Pennycook, Timothy/B-4946-2014; Jones, Lewys/R-3501-2016 OI Pennycook, Timothy/0000-0002-0008-6516; Jones, Lewys/0000-0002-6907-0731 FU EPSRC through the UK National Facility for Aberration-Corrected STEM (SuperSTEM); EPSRC [EP/K032518/1]; Division of Materials Sciences and Engineering of the U.S. department of Energy; European Union [312483] FX This research was supported by the EPSRC through the UK National Facility for Aberration-Corrected STEM (SuperSTEM) and also EPSRC grant number EP/K032518/1. Microscopy at Oak Ridge National Laboratory was sponsored by the Division of Materials Sciences and Engineering of the U.S. department of Energy. The work was partially supported by the European Union Seventh Framework Programme under Grant Agreement 312483 - ESTEEM2 (Integrated Infrastructure Initiative 13). NR 30 TC 24 Z9 24 U1 5 U2 67 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0304-3991 EI 1879-2723 J9 ULTRAMICROSCOPY JI Ultramicroscopy PD APR PY 2015 VL 151 BP 160 EP 167 DI 10.1016/j.ultramic.2014.09.013 PG 8 WC Microscopy SC Microscopy GA CD6YU UT WOS:000351237800021 PM 25458189 ER PT J AU Zaluzec, NJ AF Zaluzec, Nestor J. TI The influence of C-s/C-c correction in analytical imaging and spectroscopy in scanning and transmission electron microscopy SO ULTRAMICROSCOPY LA English DT Article; Proceedings Paper CT PICO 2015: 3rd Conference on Frontiers of Aberration Corrected Electron Microscopy CY APR 19-23, 2015 CL Vaals, NETHERLANDS DE Aberration correction; HREM; Phase contrast; Amplitude contrast; ETEM; EFTEM; AEM; EELS; XEDS; In-situ; Tomography ID ENERGY-LOSS SPECTROSCOPY; HIGH-RESOLUTION; ABERRATION CORRECTION; CHROMATIC ABERRATION; SINGLE ATOMS; TEM; PROGRESS; STEM; SPECTROMETER AB Aberration correction in scanning/transmission electron microscopy (S/TEM) owes much to the efforts of a small dedicated group of innovators. Leading that frontier has been Prof Harald Rose. To date his leadership and dynamic personality has spearheaded our ability to leave behind many of the limitations imposed by spherical aberration (C-s) in high resolution phase contrast imaging. Following shortly behind, has been the development of chromatic aberration correction (C-c) which augments those accomplishments. In this paper we will review and summarize how the combination of C-s/C-c technology enhances our ability to conduct hyperspectral imaging and spectroscopy in today's and future computationally mediated experiments in both thin as well as realistic specimens in vacuo and during in-situ/environmental experiments. (C) 2014 Elsevier B.V. All rights reserved C1 Argonne Natl Lab, Ctr Electron Microscopy, Nanosci & Technol Div, Argonne, IL 60439 USA. RP Zaluzec, NJ (reprint author), Argonne Natl Lab, Ctr Electron Microscopy, Nanosci & Technol Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM zaluzec@microscopy.com FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, at the Electron Microscopy Center in the NanoScience and Technology Division of Argonne National Laboratory [DE-AC02-06CH11357] FX This work was supported by U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, at the Electron Microscopy Center in the NanoScience and Technology Division of Argonne National Laboratory under Contract no. DE-AC02-06CH11357. Long standing collaborations and extensive discussions with J.G. Wen, D.J. Miller and R.E. Cook all of the ANL Electron Microscopy Center are gratefully acknowledged, particularly in collecting and interpreting the ACI data reproduced in this overview. NR 54 TC 1 Z9 1 U1 3 U2 28 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0304-3991 EI 1879-2723 J9 ULTRAMICROSCOPY JI Ultramicroscopy PD APR PY 2015 VL 151 BP 240 EP 249 DI 10.1016/j.ultramic.2014.09.012 PG 10 WC Microscopy SC Microscopy GA CD6YU UT WOS:000351237800029 PM 25498141 ER PT J AU Perry, DL AF Perry, Dale L. TI The tris(carbonato)dioxouranium(VI) ion: A structural model for uranium 4f(7/2), (5/2) X-ray photoelectron spectra satellite structures for oxide and oxygen coordination cores SO VACUUM LA English DT Article DE Potassium uranyl carbonate; Scanning electron microscopy (SEM); X-ray diffraction (XRD); X-ray photoelectron spectroscopy (XPS) ID URANYL CARBONATE; OXIDATION-STATES; SPECTROSCOPY; DIOXIDE; SOILS; RAMAN AB An ambient pressure synthesis of potassium tris(carbonato)dioxouranium(VI), K4UO2(CO3)(3), is reported in which a hydrolyzed uranyl salt (the first report of reacting a non-stoichiometric uranium mixture starting material to form the title compound) is reacted with potassium carbonate at ambient pressure to produce pure, high quality, large crystals of the title compound. The compound has been characterized using X-ray photoelectron spectroscopy, along with X-ray single-crystal diffraction confirmatory data that have been reported previously. Binding energies and line widths, along with the concomitant associated satellite structure of the photoelectron peaks, are reported and compared to those of similar compounds. The uranium 4f(7/2), (5/2) X-ray photoelectron lines show distinct, unique satellite features whose mechanisms of formation are discussed. (C) 2014 Elsevier Ltd. All rights reserved. C1 Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Perry, DL (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mail Stop 70A-1150, Berkeley, CA 94720 USA. EM dlperry@lbl.gov NR 35 TC 1 Z9 1 U1 1 U2 6 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0042-207X J9 VACUUM JI Vacuum PD APR PY 2015 VL 114 SI SI BP 162 EP 165 DI 10.1016/j.vacuum.2014.10.013 PG 4 WC Materials Science, Multidisciplinary; Physics, Applied SC Materials Science; Physics GA CD7CF UT WOS:000351247700028 ER PT J AU Scott, DE Yanes, Y Rothermel, BB Pilgrim, M Romanek, CS AF Scott, David E. Yanes, Yurena Rothermel, Betsie B. Pilgrim, Melissa Romanek, Christopher S. TI Efficacy of Labeling Wetlands with Enriched N-15 to Determine Amphibian Dispersal SO WETLANDS LA English DT Article DE Ambystoma; Connectivity; Isolated wetland; Metapopulation; Spiked nitrogen isotopes ID STABLE-ISOTOPE ENRICHMENT; SALAMANDER AMBYSTOMA-CALIFORNIENSE; NITROGEN CYCLING RATES; POPULATION-DYNAMICS; LARVAL DENSITY; UNITED-STATES; METAPOPULATION; CONSERVATION; CARBON; ECOLOGY AB Stable isotope enrichment techniques can aid in understanding dispersal of animals. Pond-breeding amphibians often have spatially disjunct populations that depend on immigration for persistence, yet obtaining direct estimates of dispersal rates among wetlands is challenging. We enriched aquatic mesocosms with N-15 to "mark" amphibian larvae and determine the feasibility of using enrichment techniques to study dispersal in pond-breeding amphibians. Because newly metamorphosed amphibians in mark-release-recapture studies may not be recaptured until adulthood, we estimated persistence of the N-15 enrichment signature up to 3 years post-metamorphosis. We reared larval marbled salamanders (Ambystoma opacum) in artificial mesocosms dosed with (NH4Cl)-N-15, and maintained metamorphs on unlabeled prey for 7 months to estimate the biological half life (BHL) of N-15 in tissue. Metamorphs in spiked treatments attained delta N-15 levels > 1000 times higher than reference animals (5 +/- 1aEuro degrees), and levels remained similar to 225 times higher than controls after 7 months. The average N-15 BHL was 2.49 +/- 0.24 months, indicating that the elevated signature should be discernible for a minimum of 20-28 months after metamorphosis. Our results suggest that N-15 enrichment is feasible for field studies of amphibian dispersal, as metamorphs will retain isotope-enriched tissues that persist until at least the second year of breeding. C1 [Scott, David E.; Romanek, Christopher S.] Univ Georgia, Savannah River Ecol Lab, Aiken, SC 29802 USA. [Yanes, Yurena] Univ Cincinnati, Dept Geol, Cincinnati, OH 45221 USA. [Rothermel, Betsie B.] Archbold Biol Stn, Venus, FL 33960 USA. [Pilgrim, Melissa] Univ South Carolina Upstate, Spartanburg, SC 29303 USA. RP Scott, DE (reprint author), Univ Georgia, Savannah River Ecol Lab, Aiken, SC 29802 USA. EM scott@srel.uga.edu RI Yanes, Yurena/F-3218-2010 FU Department of Energy [DE-FC09-07SR22506] FX We thank Larry Bryan, Stacey Lance, and Jim Beasley for reviews of early drafts of this manuscript, an anonymous reviewer and Robin Warne for additional comments, and Susan Walls and Ken Dodd for insights on age at maturity in southeastern amphibians. Ben Morris and Angie Tucker helped maintain metamorphosed salamanders and weigh samples for isotope analysis, and Heather Brant helped keep the instrumentation up and running. This work was partially supported by the Department of Energy under Award Number DE-FC09-07SR22506 to the University of Georgia Research Foundation. NR 56 TC 0 Z9 0 U1 0 U2 20 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0277-5212 EI 1943-6246 J9 WETLANDS JI Wetlands PD APR PY 2015 VL 35 IS 2 BP 349 EP 356 DI 10.1007/s13157-015-0624-8 PG 8 WC Ecology; Environmental Sciences SC Environmental Sciences & Ecology GA CE0XA UT WOS:000351532700012 ER PT J AU Jiang, Z Xing, Y Guo, Y Moan, T Gao, Z AF Jiang, Z. Xing, Y. Guo, Y. Moan, T. Gao, Z. TI Long-term contact fatigue analysis of a planetary bearing in a land-based wind turbine drivetrain SO WIND ENERGY LA English DT Article DE planetary bearing; contact fatigue; wind turbine drivetrain; multibody simulation; finite element; contact mechanics; Harris method; response surface method ID FINITE-ELEMENT; CRACK INITIATION; TIME-DOMAIN; LIFE; MODEL; SURFACE; STRESS; LOAD AB This paper presents an approach for performing a long-term fatigue analysis of rolling element bearings in wind turbine gearboxes. Multilevel integrated analyses were performed using the aeroservoelastic code HAWC2, the multibody dynamics code SIMPACK, the three-dimensional finite element code Calyx and a simplified lifetime prediction model for rolling contact fatigue. The National Renewable Energy Laboratory's 750kW wind turbine and its planetary bearing were studied. Design load cases, including normal production, parked and transient load cases, were considered. To obtain the internal bearing load distribution, an advanced approach combining a finite element/contact mechanics model and a response surface model were used. In addition, a traditional approach, the Harris model, was also applied for comparison. The long-term probability distribution of the bearing raceway contact pressure range was then obtained using Weibull and generalized Gamma distribution functions. Finally, we estimated the fatigue life of the bearing, discussed the differences of the methods used to obtain the bearing internal loads and analyzed the effects of the environmental conditions and load cases on the results. The Harris model may underestimate the inner raceway life by 55.7%, which can cause large load fluctuations along the raceways. The bearing fatigue life is very sensitive to the wind distribution and less affected by the transient and parked load cases. Copyright (c) 2014 John Wiley & Sons, Ltd. C1 [Jiang, Z.; Moan, T.; Gao, Z.] Norwegian Univ Sci & Technol, Dept Marine Technol, N-7491 Trondheim, Norway. [Jiang, Z.; Xing, Y.; Moan, T.; Gao, Z.] Norwegian Univ Sci & Technol, Ctr Ships & Ocean Struct, N-7491 Trondheim, Norway. [Guo, Y.] Natl Renewable Energy Lab, Natl Wind Technol Ctr, Golden, CO USA. RP Jiang, Z (reprint author), Norwegian Univ Sci & Technol, Dept Marine Technol, N-7491 Trondheim, Norway. EM zhiyu.jiang@ntnu.no FU Department of Marine Technology at the Norwegian University of Science and Technology, Trondheim, Norway; Centre for Ships and Ocean Structures at the Norwegian University of Science and Technology, Trondheim, Norway; US Department of Energy Wind and Water Power Technologies Office FX We acknowledge financial support from the Department of Marine Technology and Centre for Ships and Ocean Structures at the Norwegian University of Science and Technology, Trondheim, Norway. The gearbox and wind turbine models were provided by the GRC project at the National Renewable Energy Laboratory, CO, USA. The GRC initiative is funded by the US Department of Energy Wind and Water Power Technologies Office. The first author extends his gratitude to Dr. Wenbin Dong from Det Norsk Veritas for valuable discussions. NR 64 TC 4 Z9 4 U1 5 U2 20 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1095-4244 EI 1099-1824 J9 WIND ENERGY JI Wind Energy PD APR PY 2015 VL 18 IS 4 BP 591 EP 611 DI 10.1002/we.1713 PG 21 WC Energy & Fuels; Engineering, Mechanical SC Energy & Fuels; Engineering GA CD6BC UT WOS:000351172400002 ER PT J AU Guo, Y Keller, J LaCava, W AF Guo, Yi Keller, Jonathan LaCava, William TI Planetary gear load sharing of wind turbine drivetrains subjected to non-torque loads SO WIND ENERGY LA English DT Article DE wind turbine; load sharing; planetary gear; non-torque load; pitching moment; bearing clearance ID BEHAVIOR AB An analytical formulation was developed to estimate the load-sharing and planetary loads of a three-point suspension wind turbine drivetrain considering the effects of non-torque loads, gravity and bearing clearance. A three-dimensional dynamic drivetrain model that includes mesh stiffness variation, tooth modifications and gearbox housing flexibility was also established to investigate gear tooth load distribution and non-linear tooth and bearing contact of the planetary gears. These models were validated with experimental data from the National Renewable Energy Laboratory's Gearbox Reliability Collaborative. Non-torque loads and gravity induce fundamental excitations in the rotating carrier frame, which can increase gearbox loads and disturb load sharing. Clearance in the carrier bearings reduces the bearing stiffness significantly. This increases the amount of pitching moment transmitted from the rotor to the gear meshes and disturbs the planetary load share, thereby resulting in edge loading. Edge loading increases the likelihood of tooth pitting and planet-bearing fatigue, leading to reduced gearbox life. Additionally, at low-input torque, the planet-bearing loads are often less than the minimum recommended load and thus susceptible to skidding. Copyright (c) 2014 John Wiley & Sons, Ltd. C1 [Guo, Yi; Keller, Jonathan] Natl Renewable Energy Lab, Natl Wind Technol Ctr, Golden, CO USA. [LaCava, William] Univ Massachusetts, Amherst, MA 01003 USA. RP Keller, J (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM jonathan.keller@nrel.gov FU US Department of Energy [DE-AC36-08GO28308]; NREL FX This work was supported by the US Department of Energy under contract no. DE-AC36-08GO28308 with the NREL. NR 30 TC 4 Z9 4 U1 6 U2 28 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1095-4244 EI 1099-1824 J9 WIND ENERGY JI Wind Energy PD APR PY 2015 VL 18 IS 4 BP 757 EP 768 DI 10.1002/we.1731 PG 12 WC Energy & Fuels; Engineering, Mechanical SC Energy & Fuels; Engineering GA CD6BC UT WOS:000351172400012 ER PT J AU Tucker, JD Miller, MK Young, GA AF Tucker, J. D. Miller, M. K. Young, G. A. TI Assessment of thermal embrittlement in duplex stainless steels 2003 and 2205 for nuclear power applications SO ACTA MATERIALIA LA English DT Article DE Duplex stainless steels; 475 degrees C embrittlement; Spinodal decomposition; Atom probe tomography ID ATOM-PROBE; EXPONENT AB Duplex stainless steels are desirable for use in power generation systems because of their attractive combination of strength, corrosion resistance and cost. However, thermal embrittlement at intermediate homologous temperatures of similar to 475 degrees C and below, limits upper service temperatures for many applications. New lean grade duplex alloys have improved thermal stability over standard grades and potentially increase the upper service temperature or the lifetime at a given temperature for this class of material. The present work compares the thermal stability of lean grade, alloy 2003, to standard grade, alloy 2205, through a series of isothermal agings between 260 degrees C and 482 degrees C for times between 1 and 10,000 h. Aged samples were characterized by changes in microhardness and impact toughness. Additionally, atom probe tomography was performed to illustrate the evolution of the alpha-alpha' phase separation in both alloys at select conditions. Atom probe tomography confirmed that phase separation occurs via spinodal decomposition for both alloys, and identified the presence of Ni-Cu-Si-Mn-P clusters in alloy 2205, which may contribute to the embrittlement of this alloy. The impact toughness model predictions for the upper service temperature show that alloy 2003 may be viable for use in 288 degrees C applications for 80-year service lifetimes based on a Charpy V-notch criteria of 47 J at room temperature. In comparison, alloy 2205 should be limited to 260 degrees C applications for the same room temperature toughness of 47 J. (C) 2014 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Tucker, J. D.] Oregon State Univ, Corvallis, OR 97331 USA. [Miller, M. K.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Young, G. A.] Knolls Atom Power Lab, Niskayuna, NY 12309 USA. RP Tucker, JD (reprint author), Oregon State Univ, 204 Rogers Hall, Corvallis, OR 97331 USA. EM julie.tucker@oregonstate.edu FU ORNL's Center for Nanophase Materials Sciences (CNMS) - Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy FX The authors gratefully acknowledge the assistance of the following contributors: Ms. Kathy Powers at Oak Ridge National Laboratory for sample preparation and atom probe analysis, and Ms. Chelsea Ehlert at Rensselaer Polytechnic Institute for microhardness testing; at the Knolls Atomic Power Laboratory: Dr. Dan R. Eno for statistical analysis, and Mr. Joe Badalucco for the metallography, impact toughness and microhardness testing. APT research was performed as part of a user project supported by ORNL's Center for Nanophase Materials Sciences (CNMS), which is sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. NR 22 TC 14 Z9 16 U1 4 U2 34 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD APR 1 PY 2015 VL 87 BP 15 EP 24 DI 10.1016/j.actamat.2014.12.012 PG 10 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA CC6ZO UT WOS:000350517700003 ER PT J AU Boegelein, T Dryepondt, SN Pandey, A Dawson, K Tatlock, GJ AF Boegelein, Thomas Dryepondt, Sebastien N. Pandey, Amit Dawson, Karl Tatlock, Gordon J. TI Mechanical response and deformation mechanisms of ferritic oxide dispersion strengthened steel structures produced by selective laser melting SO ACTA MATERIALIA LA English DT Article DE Oxide dispersion strengthened alloys; Rapid prototyping; Tensile testing; Anisotropy; Transmission electron microscopy ID ODS ALLOYS; PM2000; BEHAVIOR; POWDER; IRON AB Oxide dispersion strengthened (ODS) ferritic steels typically contain a fine dispersion of nanoscopic Y(Al, Ti) oxides, leading to an improvement in mechanical and physical properties. A rapid prototyping technique, selective laser melting (SLM), was successfully applied to consolidate as-mechanically alloyed ODS-PM2000 (Fe-19Cr-5.5Al-0.5Ti-0.5Y(2)O(3); all wt.%) powder to fabricate solid and thin-walled builds of different thickness. This work is intended to act as a first study to investigate the tensile response of such configurations at room temperature, using miniaturized test specimens along and perpendicular to the growth direction. The 0.2% offset yield strength of as-grown wall builds was inferior to conventional PM2000 alloy (recrystallized), but could be significantly increased by conducting post-build heat treatments. Young's modulus and yield strength showed anisotropy and were enhanced when testing perpendicular to the build growth direction. Electron backscatter diffraction revealed a strong [0 0 1] fibre texture along the growth direction, which explains the anisotropic behaviour. Additionally, studies on the morphology of the individual fracture surfaces, the grain structure of the cross-section near this region and the size distribution of ODS particles in such builds were conducted. A fine dispersion of precipitates was retained in all SLM builds, and findings suggest that a certain amount of Y is probably still in atomic solution in the as-grown condition and forms new small nanoscopic dispersoids during annealing, which lead to enhanced strengthening. (C) 2015 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Boegelein, Thomas; Dawson, Karl; Tatlock, Gordon J.] Univ Liverpool, Sch Engn, Ctr Mat & Struct, Liverpool L69 3GH, Merseyside, England. [Boegelein, Thomas; Dryepondt, Sebastien N.; Pandey, Amit] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Boegelein, T (reprint author), Univ Liverpool, Sch Engn, Ctr Mat & Struct, Liverpool L69 3GH, Merseyside, England. EM t.boegelein@liv.ac.uk OI Dawson, Karl/0000-0003-3249-8328 FU Advanced Research Materials (ARM) Programme, U.S. Department of Energy, Office of Fossil Energy; EPSRC grant (Materials for Fusion and Fission Power) [EP/H018921/1] FX The builds were produced in the Manufacturing Science and Engineering Research Centre at the University of Liverpool, led by Dr. C.J. Sutcliffe. Members of the group, in particular Dr. J. Singh and Dr. J. Robinson, gave valuable input. Thanks to Dr. G. Pimentel, from the Centro Nacional De Investigaciones Metalurgicas in Madrid, Spain, for providing a recipe for an etchant to reveal the grain structure of the present builds. We are grateful for financial support of the work through the Advanced Research Materials (ARM) Programme, U.S. Department of Energy, Office of Fossil Energy, managed by U.T.-Battelle, LLC, and funding by EPSRC grant EP/H018921/1 (Materials for Fusion and Fission Power). NR 52 TC 10 Z9 10 U1 9 U2 92 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD APR 1 PY 2015 VL 87 BP 201 EP 215 DI 10.1016/j.actamat.2014.12.047 PG 15 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA CC6ZO UT WOS:000350517700020 ER PT J AU Xiao, HY Weber, WJ Zhang, Y Zu, XT AF Xiao, H. Y. Weber, W. J. Zhang, Y. Zu, X. T. TI Ab initio molecular dynamics simulations of ion-solid interactions in zirconate pyrochlores SO ACTA MATERIALIA LA English DT Article DE Computer simulation; Zirconate pyrochlores; Radiation effects; Charge transfer ID GADOLINIUM ZIRCONATE; RADIATION-DAMAGE; WASTE FORM; PSEUDOPOTENTIALS; IMMOBILIZATION; PLUTONIUM; GD2TI2O7; OXIDES; SM AB In this study, an ab initio molecular dynamics method is employed to study low energy recoil events in zirconate pyrochlores (A(2)Zr(2)O(7), A = La, Nd and Sm). It shows that both cations and anions in Nd2Zr2O7 and Sm2Zr2O7 are generally more likely to be displaced than those in La2Zr2O7. The damage end states mainly consist of Frenkel pair defects, and the Frenkel pair formation energies in Nd2Zr2O7 and Sm2Zr2O7 are lower than those in La2Zr2O7. These results suggest that the order disorder structural transition more easily occurs in Nd2Zr2O7 and Sm2Zr2O7 resulting in a defect-fluorite structure, which agrees well with experimental observations. Our calculations indicate that oxygen migration from 48f and 8b to 8a sites is dominant under low energy irradiation. A number of new defects, including four types of cation Frenkel pairs and six types of anion Frenkel pairs, are revealed by ab initio molecular dynamics simulations. The present results may help to advance the fundamental understanding of the irradiation response behavior of zirconate pyrochlores. (C) 2015 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Xiao, H. Y.; Zu, X. T.] Univ Elect Sci & Technol China, Sch Phys Elect, Chengdu 610054, Peoples R China. [Weber, W. J.; Zhang, Y.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Weber, W. J.; Zhang, Y.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Zu, X. T.] Univ Elect Sci & Technol China, Inst Fundamental & Frontier Sci, Chengdu 610054, Peoples R China. RP Xiao, HY (reprint author), Univ Elect Sci & Technol China, Sch Phys Elect, Chengdu 610054, Peoples R China. EM hyxiao@uestc.edu.cn RI Weber, William/A-4177-2008 OI Weber, William/0000-0002-9017-7365 FU scientific research starting funding of University of Electronic Science and Technology of China [Y02002010401085]; NSAF Joint Foundation of China [U1330103]; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division FX H.Y. Xiao was supported by the scientific research starting funding of University of Electronic Science and Technology of China (Grant No. Y02002010401085) and by the NSAF Joint Foundation of China (Grant No. U1330103). W.J. Weber and Y. Zhang were supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. The theoretical calculations were performed using the supercomputer resources at TianHe-1 located at National Supercomputer Center in Tianjin. NR 37 TC 5 Z9 5 U1 4 U2 49 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD APR 1 PY 2015 VL 87 BP 273 EP 282 DI 10.1016/j.actamat.2015.01.019 PG 10 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA CC6ZO UT WOS:000350517700027 ER PT J AU Barabash, RI Barabash, OM Popov, D Shen, GY Park, CY Yang, WG AF Barabash, Rozaliya I. Barabash, Oleg M. Popov, Dmitry Shen, Guoyin Park, Changyong Yang, Wenge TI Multiscale twin hierarchy in NiMnGa shape memory alloys with Fe and Cu SO ACTA MATERIALIA LA English DT Article DE Shape memory alloys; X-ray microdiffraction; Twin boundaries; Scanning electron microscopy; Multiscale structure ID GA SINGLE-CRYSTALS; MAGNETIC-FIELD; NEUTRON-DIFFRACTION; MARTENSITIC PHASES; TRANSFORMATION; DEFORMATION; BOUNDARIES; MOTION AB X-ray microdiffraction and scanning electron microscopy studies reveal 10 M martensitic structure with a highly correlated multiscale twin hierarchy organization in NiMnGaFeCu shape memory alloys. High compatibility is found at the twin interfaces resulting in a highly correlated twinned lattice orientation across several laminate levels. The lattice unit cell is described as monoclinic I-centered with a = 4.28 angstrom, b = 4.27 angstrom, c = 5.40 angstrom, gamma = 78.5 degrees. The modulation is found parallel to the b axis. Thin tapered needle-like lamellae and branching are observed near the twin boundaries. Published by Elsevier Ltd. on behalf of Acta Materialia Inc. C1 [Barabash, Rozaliya I.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Barabash, Oleg M.] Univ Tennessee, Knoxville, TN 37996 USA. [Popov, Dmitry; Shen, Guoyin; Park, Changyong] Carnegie Inst Sci, Geophys Lab, HPCAT, Argonne, IL 60439 USA. [Yang, Wenge] Ctr High Pressure Sci & Technol Adv Res HPSTAR, Shanghai 201203, Peoples R China. RP Barabash, RI (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. EM rbarabas@utk.edu; dpopov@carnegiescience.edu RI Park, Changyong/A-8544-2008 OI Park, Changyong/0000-0002-3363-5788 FU Laboratory Directed Research and Development Program of Oak Ridge National Laboratory; ORNL's Center for Nanophase Materials Sciences; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; DOE-NNSA [DE-NA0001974]; DOE-BES [DE-FG02-99ER45775]; NSF; DOE Office of Science by Argonne National Laboratory [DE-AC02-06CH11357] FX Research sponsored by the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy. Research conducted as part of a user project supported by ORNL's Center for Nanophase Materials Sciences, which is sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. HPCAT operations are supported by DOE-NNSA under Award No. DE-NA0001974 and DOE-BES under Award No. DE-FG02-99ER45775, with partial instrumentation funding by NSF. The Advanced Photon Source is a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. NR 45 TC 1 Z9 1 U1 4 U2 49 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD APR 1 PY 2015 VL 87 BP 344 EP 349 DI 10.1016/j.actamat.2015.01.010 PG 6 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA CC6ZO UT WOS:000350517700033 ER PT J AU Fleischmann, E Miller, MK Affeldt, E Glatzel, U AF Fleischmann, Ernst Miller, Michael K. Affeldt, Ernst Glatzel, Uwe TI Quantitative experimental determination of the solid solution hardening potential of rhenium, tungsten and molybdenum in single-crystal nickel-based superalloys SO ACTA MATERIALIA LA English DT Article DE Solid solution; Single crystal; Creep; Nickel-based superalloys; Rhenium ID STACKING-FAULT ENERGY; NI-BASED SUPERALLOYS; CREEP-PROPERTIES; CR ALLOYS; TEMPERATURE ALLOYS; MATRIX; MICROSTRUCTURE; MICROSCOPY; BEHAVIOR; DESIGN AB The solid-solution hardening potential of the refractory elements rhenium, tungsten and molybdenum in the matrix of single-crystal nickel-based superalloys was experimentally quantified. Single-phase alloys with the composition of the nickel solid-solution matrix of superalloys were cast as single crystals, and tested in creep at 980 degrees C and 30-75 MPa. The use of single-phase single-crystalline material ensures very clean data because no grain boundary or particle strengthening effects interfere with the solid-solution hardening. This makes it possible to quantify the amount of rhenium, tungsten and molybdenum necessary to reduce the creep rate by a factor of 10. Rhenium is more than two times more effective for matrix strengthening than either tungsten or molybdenum. The existence of rhenium clusters as a possible reason for the strong strengthening effect is excluded as a result of atom probe tomography measurements. If the partitioning coefficient of rhenium, tungsten and molybdenum between the gamma matrix and the gamma' precipitates is taken into account, the effectiveness of the alloying elements in two-phase superalloys can be calculated and the rhenium effect can be explained. (C) 2014 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Fleischmann, Ernst; Glatzel, Uwe] Univ Bayreuth, Met & Alloys, D-95447 Bayreuth, Germany. [Miller, Michael K.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Affeldt, Ernst] MTU Aero Engines AG, D-80995 Munich, Germany. RP Glatzel, U (reprint author), Univ Bayreuth, Met & Alloys, Ludwig Thoma Str 36b, D-95447 Bayreuth, Germany. EM uwe.glatzel@uni-bayreuth.de FU Bundesministerium fur Wirtschaft und Technologie; MTU Aero Engines AG [Lufo 4/3 - AP2.3] FX Funding of this project by the Bundesministerium fur Wirtschaft und Technologie and MTU Aero Engines AG within Lufo 4/3 - AP2.3: "Kostengunstiger Re-freier SX-Werkstoff" is gratefully acknowledged. Atom probe tomography (M.K.M.) was conducted at the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. NR 46 TC 9 Z9 10 U1 10 U2 31 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD APR 1 PY 2015 VL 87 BP 350 EP 356 DI 10.1016/j.actamat.2014.12.011 PG 7 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA CC6ZO UT WOS:000350517700034 ER PT J AU Cai, S Sehaffer, JE Ren, Y Daymond, MR AF Cai, Song Sehaffer, Jeremy E. Ren, Yang Daymond, Mark R. TI Discovery of a < 210 >-fiber texture in medical-grade metastable beta titanium wire SO ACTA MATERIALIA LA English DT Article DE Beta titanium; 332 Twinning; Polycrystal plasticity modeling; Synchrotron X-ray diffraction; Wire texture ID SPINAL FIXATION APPLICATIONS; CHANGEABLE YOUNGS MODULUS; ALLOY SINGLE-CRYSTALS; ZIRCONIUM ALLOYS; PHASE-STABILITY; DEFORMATION; STRAIN; POLYCRYSTALS; BEHAVIOR AB The texture and phase evolution of metastable beta-III Ti alloy wires, produced in a medical-grade wire-processing facility, are examined via synchrotron X-ray diffraction. The texture development in the beta-phase was interpreted by a simple viscoplastic self-consistent (VPSC) modeling approach. Both the stress-induced martensite and stress-induced omega phase transformations are observed during the early stage of cold deformation. The < 1 1 0 >(beta) texture is gradually replaced by the < 2 1 0 >(beta) texture at cold work levels above 50% total area reduction or equivalently 0.70 axial true strain. Formation of the < 2 1 0 >(beta)-fiber from the combined activity of {1 1 2} and {3 3 2} twinning plus conventional slip is observed and may not directly depend upon the stress-induced phase per se. According to the VPSC model, similar texture should occur in other metastable beta-Ti alloys subjected to similar wire processing. These data should help inform process-structure-function towards better wire design in titanium-based medical devices. (C) 2015 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Cai, Song; Sehaffer, Jeremy E.] Ft Wayne Met Res Prod Corp, Ft Wayne, IN 46809 USA. [Ren, Yang] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Daymond, Mark R.] Queens Univ, Dept Mech & Mat Engn, Kingston, ON K7L 3N6, Canada. RP Sehaffer, JE (reprint author), Ft Wayne Met Res Prod Corp, 9609 Ardmore Ave, Ft Wayne, IN 46809 USA. EM Jeremy_schaffer@fwmetals.com OI Daymond, Mark/0000-0001-6242-7489 FU U.S. Department of Energy, Office of Science [DE-AC02-06CH11357]; Fort Wayne Metals FX Use of the synchrotron X-ray at APS was granted by the U.S. Department of Energy, Office of Science, under Contract No. DE-AC02-06CH11357. Data analysis was performed using FIT2D and MAUD software. The VPSC modeling code was provided by C. Tome. C. Yu (Ph.D. student) for X-ray diffraction and P. Sims for sample production. Funding and support from Fort Wayne Metals towards this project is acknowledged and greatly appreciated. NR 37 TC 3 Z9 3 U1 2 U2 13 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD APR 1 PY 2015 VL 87 BP 390 EP 398 DI 10.1016/j.actamat.2014.12.035 PG 9 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA CC6ZO UT WOS:000350517700037 ER PT J AU Tourret, D Karma, A AF Tourret, D. Karma, A. TI Multi-scale dendritic needle network model of alloy solidification (vol 61, pg 6474, 2013) SO ACTA MATERIALIA LA English DT Correction C1 [Tourret, D.; Karma, A.] Northeastern Univ, Dept Phys, Boston, MA 02115 USA. [Tourret, D.; Karma, A.] Northeastern Univ, Ctr Interdisciplinary Res Complex Syst, Boston, MA 02115 USA. [Tourret, D.] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. RP Tourret, D (reprint author), Northeastern Univ, Dept Phys, Boston, MA 02115 USA. EM dtourret@lanl.gov; a.karma@neu.edu NR 1 TC 2 Z9 2 U1 1 U2 18 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD APR 1 PY 2015 VL 87 BP 411 EP 411 DI 10.1016/j.actamat.2015.01.026 PG 1 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA CC6ZO UT WOS:000350517700039 ER PT J AU Scheele, RD Wend, CF AF Scheele, Randall D. Wend, Christopher F. TI Solidification and stabilization of silver mordenite used to control radioiodine emissions from Hanford's Waste Treatment Plant SO ANNALS OF NUCLEAR ENERGY LA English DT Article DE Reduced-silver mordenite; Silver mordenite; Silver waste land disposal; Silver waste solidification and stabilization; Cement immobilization; Targeted precipitation agent ID CEMENT AB The United States Department of Energy is building the Hanford Waste Treatment and Immobilization Plant (WTP) in south-central Washington State to immobilize a portion of the stored high-level radioactive wastes generated by decades of producing nuclear defense material. To comply with United States Environmental Protection Agency (EPA) and Washington State air emission regulations, the WTP is planning to use reduced silver mordenite to control releases of any volatilized waste constituent radioiodine (I-129 t(1/2) = 1.7 x 10(7) a). Because the EPA and Washington State have designated silver as a hazardous or dangerous waste constituent, the disposal form for the waste reduced silver mordenite must comply with their land disposal regulations. We used the mandated EPA Toxic Characteristic Leach Procedure to evaluate and qualify a disposal form for the waste reduced-silver mordenite. Our development effort resulted in a regulation-compliant disposal form which used cast American Society for Testing and Materials (ASTM) Portland Type III cement modified to include calcium iodide to solidify and stabilize the reduced-silver mordenite and control silver release to regulatory levels. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Scheele, Randall D.] Battelle Pacific NW Div, Richland, WA 99352 USA. [Wend, Christopher F.] Northwest Agr Prod, Pasco, WA 99301 USA. RP Scheele, RD (reprint author), Battelle Pacific NW Div, POB 999,Battelle Blvd, Richland, WA 99352 USA. EM randall.scheele@pnnl.gov; chrisw@nap-chem.com FU Bechtel National FX We thank Bechtel National for their financial support. We thank and acknowledge W.C. Buchmiller, A.E. Kozelisky, and R.L. Sell, who prepared the various silver mordenites and the grouted zeolites that were evaluated by the TestAmerica laboratory using EPA's TCLP procedure. We thank C.H. Delegard for his technical review and W.C. Cosby, RE. Schrempf, and T.M. Scheele for their editorial review. NR 31 TC 4 Z9 4 U1 3 U2 18 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0306-4549 J9 ANN NUCL ENERGY JI Ann. Nucl. Energy PD APR PY 2015 VL 78 BP 40 EP 48 DI 10.1016/j.anucene.2014.12.019 PG 9 WC Nuclear Science & Technology SC Nuclear Science & Technology GA CD0QQ UT WOS:000350779400006 ER PT J AU Fisk, WJ AF Fisk, William J. TI Review of some effects of climate change on indoor environmental quality and health and associated no-regrets mitigation measures SO BUILDING AND ENVIRONMENT LA English DT Article DE Building; Climate change; Health; Indoor air quality; Indoor environmental quality; Mitigation ID SOUTHERN CALIFORNIA WILDFIRES; OZONE-RELATED MORTALITY; REDUCING RELATIVE-HUMIDITY; PARTICULATE AIR-POLLUTION; CASE-CROSSOVER ANALYSIS; HEAT-RELATED MORTALITY; SHORT-TERM MORTALITY; SEA-LEVEL RISE; UNITED-STATES; PUBLIC-HEALTH AB This paper reviews the potential health consequences of changes in climate that affect indoor environments, with an emphasis on residential environments in the U.S. and Europe. These changes in climate, include increases in the frequency and severity of heat waves, severe storms coupled with sea level rise, and wildfires, plus increases in urban airborne ozone. The potential for adverse health effects is substantial. Examples of projected effects include a doubling of heat-related deaths, increased hospitalizations for asthma, pneumonia, and cardiovascular effects during wildfires, and increased mortality and hospitalizations associated with ozone. The associated adverse exposures occur, to a significant extent, indoors. The adverse health effects will be substantially mediated by features of buildings, particularly of homes where people, particularly those most susceptible, spend the largest amount of time. Changes to buildings, or to building operations, are identified that could reduce the projected adverse health effects of climate change. Examples include improved roof insulation, roof coatings that reflect more solar energy, and more air conditioning to reduce indoor overheating. Improved particle filtration systems could reduce the health effects of particles from wildfires. Some of these measures will also reduce building energy use and the associated emissions of greenhouse gases. Most of these measures would improve health irrespective of climate change. Improvements in building energy efficiency in order to mitigate climate change, has to potential to either improve or worsen indoor environmental quality and health. (C) 2015 Elsevier Ltd. All rights reserved. C1 Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Indoor Environm Grp, Berkeley, CA 94720 USA. RP Fisk, WJ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Indoor Environm Grp, 90R3058,1 Cyclotron Rd, Berkeley, CA 94720 USA. EM wjfisk@lbl.gov FU Indoor Environments Division, Office of Radiation and Indoor Air of the U.S. Environmental Protection Agency (EPA) [DW- 89-92337001]; U.S. Department of Energy [DW- 89-92337001, DE-AC02-05CH11231] FX This study was funded through interagency agreement DW- 89-92337001 between the Indoor Environments Division, Office of Radiation and Indoor Air of the U.S. Environmental Protection Agency (EPA) and the U. S. Department of Energy under contract DE-AC02-05CH11231, to develop an IAQ Scientific Findings Resource Bank (see www.iaqscience.lbl.gov). Conclusions in this paper are those of the author and not necessarily those of the U.S. EPA. The author thanks Greg Brunner for program management, and Greg Brunner, William Nazaroff, Rengie Chan, and Laura Kolb for reviewing a draft of a document on which this paper is based. NR 122 TC 5 Z9 5 U1 5 U2 56 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-1323 EI 1873-684X J9 BUILD ENVIRON JI Build. Environ. PD APR PY 2015 VL 86 BP 70 EP 80 DI 10.1016/j.buildenv.2014.12.024 PG 11 WC Construction & Building Technology; Engineering, Environmental; Engineering, Civil SC Construction & Building Technology; Engineering GA CC7CC UT WOS:000350524300007 ER PT J AU Rose, CM Bazjanac, V AF Rose, Cody M. Bazjanac, Vladimir TI An algorithm to generate space boundaries for building energy simulation SO ENGINEERING WITH COMPUTERS LA English DT Article AB We provide an algorithm based on graph theory to convert a three-dimensional architectural building model without defined thermal space boundaries into geometry suitable for import into a whole-building energy performance simulation engine such as EnergyPlus. Our algorithm expects input specified as an Industry Foundation Classes model, accepts a wide variety of input geometry, and is capable of accounting for a building's construction material configuration as well as its geometry. The described approach is limited to solid-to-solid heat exchange; solid-to-fluid and fluid-to-fluid heat exchanges are not considered. We analyze the performance of our algorithm on some test building models. C1 [Rose, Cody M.; Bazjanac, Vladimir] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Rose, CM (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd,MS90R3111, Berkeley, CA 94720 USA. EM rosecodym@gmail.com; v_bazjanac@lbl.gov FU Office of Building Technology, Building Technologies Program of the U.S. Department of Energy [DE-AC02-05CH11231] FX The authors would like to thank Natasa Mrazovic and Junia Compostella di Sanguinetto for their tireless generation of test cases and hunting of bugs, Dr. Tobias Maile for his thoughts and contributions to the predecessor of this work, and Dr. James O'Donnell for his advice during the entire project. This work was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Building Technology, Building Technologies Program of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 14 TC 1 Z9 1 U1 1 U2 1 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0177-0667 EI 1435-5663 J9 ENG COMPUT-GERMANY JI Eng. Comput. PD APR PY 2015 VL 31 IS 2 BP 271 EP 280 DI 10.1007/s00366-013-0347-5 PG 10 WC Computer Science, Interdisciplinary Applications; Engineering, Mechanical SC Computer Science; Engineering GA CD6MT UT WOS:000351203900005 ER PT J AU Kuske, CR Hesse, CN Challacombe, JF Cullen, D Herr, JR Mueller, RC Tsang, A Vilgalys, R AF Kuske, Cheryl R. Hesse, Cedar N. Challacombe, Jean F. Cullen, Daniel Herr, Joshua R. Mueller, Rebecca C. Tsang, Adrian Vilgalys, Rytas TI Prospects and challenges for fungal metatranscriptomics of complex communities SO FUNGAL ECOLOGY LA English DT Editorial Material ID TRANSCRIPTOME; METAGENOMICS C1 [Kuske, Cheryl R.; Hesse, Cedar N.; Challacombe, Jean F.; Mueller, Rebecca C.] Los Alamos Natl Lab, Biosci Div, Los Alamos, NM 87545 USA. [Cullen, Daniel] Univ Wisconsin, USDA, Forest Prod Lab, Madison, WI 53726 USA. [Herr, Joshua R.] Michigan State Univ, Dept Microbiol & Mol Genet, E Lansing, MI 48824 USA. [Tsang, Adrian] Concordia Univ, Ctr Struct & Funct Genom, Montreal, PQ H4B 1R6, Canada. [Vilgalys, Rytas] Duke Univ, Biol Sci, Durham, NC 27708 USA. RP Kuske, CR (reprint author), Los Alamos Natl Lab, Biosci Div, M888, Los Alamos, NM 87545 USA. OI Herr, Joshua/0000-0003-3425-292X NR 15 TC 7 Z9 7 U1 1 U2 29 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 1754-5048 EI 1878-0083 J9 FUNGAL ECOL JI Fungal Ecol. PD APR PY 2015 VL 14 BP 133 EP 137 DI 10.1016/j.funeco.2014.12.005 PG 5 WC Ecology; Mycology SC Environmental Sciences & Ecology; Mycology GA CD2VE UT WOS:000350936300016 ER PT J AU Justus, AL AF Justus, Alan L. TI DERIVATION OF A SIMPLE RELATIONSHIP BETWEEN PULSED AND STEADY-STATE DOSE LIMITS DUE TO GENERAL RECOMBINATION WITHIN AIR-FILLED IONIZATION CHAMBERS SO HEALTH PHYSICS LA English DT Article DE accelerators; dose assessment; ionization chambers; photons ID COLLECTION AB This paper discusses various calculational and measurement methods involved with general recombination losses of air-filled ionization chambers exposed to either steady-state or pulsed photon fields. Derived therefrom is a simple relationship between the pulsed and steady-state cases that allows the determination of expected pulsed-field losses from steady-state loss measurements within, for instance, typical Cs-137 calibration fields. Several examples are provided to illustrate each calculational and measurement method, as well as the newly derived relationship. C1 Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Justus, AL (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM ajustus@lanl.gov FU U.S. Department of Energy [DE-AC52-06NA25396] FX The author would like to thank Tom McLean, LANL, and the anonymous reviewers for their very helpful comments. This work has been authored by an employee of Los Alamos National Security, LLC, operator of the Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting this work for publication, acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce this work, or allow others to do so for United States Government purposes. NR 8 TC 0 Z9 0 U1 0 U2 2 PU LIPPINCOTT WILLIAMS & WILKINS PI PHILADELPHIA PA TWO COMMERCE SQ, 2001 MARKET ST, PHILADELPHIA, PA 19103 USA SN 0017-9078 EI 1538-5159 J9 HEALTH PHYS JI Health Phys. PD APR PY 2015 VL 108 IS 4 BP 451 EP 461 DI 10.1097/HP.0000000000000222 PG 11 WC Environmental Sciences; Public, Environmental & Occupational Health; Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical Imaging SC Environmental Sciences & Ecology; Public, Environmental & Occupational Health; Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical Imaging GA CC9AX UT WOS:000350660900007 PM 25706139 ER PT J AU Hawkley, G Whicker, J Harris, J AF Hawkley, Gavin Whicker, Jeffrey Harris, Jason TI OBSERVATIONS ON USING INSIDE AIR CONCENTRATIONS AS A PREDICTOR OF OUTSIDE AIR CONCENTRATIONS SO HEALTH PHYSICS LA English DT Article DE air sampling; atmospheric testing; dose assessment; environmental transport AB Excavations of radiological material were performed within confined structures with known operational parameters, such as a filtered exhaust system with known filtration efficiency. Given the known efficiency, the assumption could be made that the air concentrations of radioactivity measured outside the structure would be proportional to the air concentrations measured inside the structure. To investigate this assumption, the inside concentration data was compared with the outside concentration data. The correlation of the data suggested that the inside concentrations were not a good predictor of the outside concentrations. This poor correlation was deemed to be a result of operational unknowns within the structures. C1 [Hawkley, Gavin; Harris, Jason] Idaho State Univ, Dept Nucl Engn & Hlth Phys, Pocatello, ID 83209 USA. [Hawkley, Gavin; Whicker, Jeffrey] Idaho Natl Lab, Idaho Falls, ID 83415 USA. Los Alamos Natl Lab, Los Alamos, NM 87544 USA. RP Hawkley, G (reprint author), Idaho Natl Lab, Idaho Falls, ID 83415 USA. EM hawkgavi@isu.edu NR 4 TC 0 Z9 0 U1 0 U2 1 PU LIPPINCOTT WILLIAMS & WILKINS PI PHILADELPHIA PA TWO COMMERCE SQ, 2001 MARKET ST, PHILADELPHIA, PA 19103 USA SN 0017-9078 EI 1538-5159 J9 HEALTH PHYS JI Health Phys. PD APR PY 2015 VL 108 IS 4 BP 465 EP 467 DI 10.1097/HP.0000000000000223 PG 3 WC Environmental Sciences; Public, Environmental & Occupational Health; Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical Imaging SC Environmental Sciences & Ecology; Public, Environmental & Occupational Health; Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical Imaging GA CC9AX UT WOS:000350660900009 PM 25706141 ER PT J AU Chandola, N Lebensohn, RA Cazacu, O Revil-Baudard, B Mishra, RK Barlat, F AF Chandola, Nitin Lebensohn, Ricardo A. Cazacu, Oana Revil-Baudard, Benoit Mishra, Raja K. Barlat, Frederic TI Combined effects of anisotropy and tension-compression asymmetry on the torsional response of AZ31 Mg SO INTERNATIONAL JOURNAL OF SOLIDS AND STRUCTURES LA English DT Article DE Orthotropy; Strength differential effects; Twinning; Swift effects; Magnesium (AZ31) ID MAGNESIUM ALLOY AZ31B; FREE-END TORSION; NONLINEAR MECHANICAL RESPONSE; LENGTH CHANGES; TEXTURE DEVELOPMENT; ZIRCONIUM ALLOYS; METALS; DEFORMATION; EVOLUTION; BEHAVIOR AB In this paper it is demonstrated that only by accounting for the combined effects of anisotropy and tension-compression asymmetry at polycrystal level, it is possible to explain and accurately predict the room-temperature torsional response of a strongly textured AZ31 Mg material. This is shown by using two modeling frameworks, namely: a viscoplastic self-consistent (VPSC) polycrystal model, and a macroscopic plasticity model based on an yield criterion, developed by Cazacu et al. (2006), that accounts for both orthotropy and tension-compression asymmetry in plastic flow. It is shown that unlike Hill's (1948) criterion, the latter macroscopic criterion quantitatively predicts the experimental results, namely: that the sample with axial direction along the rolling direction contracts, while the sample with axial direction along the normal direction elongates. Moreover, it is demonstrated that these experimentally observed axial strain effects can be quantitatively predicted with the VPSC polycrystal model, only if both slip and twinning are considered operational at single crystal level. On the other hand, if it is assumed that the plastic deformation is fully accommodated by crystallographic slip, the axial strains predicted by VPSC are very close with that predicted with Hill (1948) criterion, which largely underestimates the measured axial strain in the rolling direction, and predicts zero axial strain in the normal direction. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Chandola, Nitin; Cazacu, Oana; Revil-Baudard, Benoit] Univ Florida, Dept Mech & Aerosp Engn, REEF, Shalimar, FL 32579 USA. [Lebensohn, Ricardo A.] Los Alamos Natl Lab, Mat Sci & Technol Div, Los Alamos, NM 87545 USA. [Mishra, Raja K.] Gen Motors Res & Dev Ctr, Warren, MI 48090 USA. [Barlat, Frederic] Pohang Univ Sci & Technol, Grad Inst Ferrous Technol, Pohang, South Korea. RP Cazacu, O (reprint author), Univ Florida, Dept Mech & Aerosp Engn, REEF, Shalimar, FL 32579 USA. EM cazacu@reef.ufl.edu RI Lebensohn, Ricardo/A-2494-2008; Cazacu, Oana/L-4635-2016; Revil-Baudard, Benoit/L-5576-2016; OI Lebensohn, Ricardo/0000-0002-3152-9105; Cazacu, Oana/0000-0002-2499-9096; Revil-Baudard, Benoit/0000-0001-8682-5035; Barlat, Frederic/0000-0002-4463-3454 NR 33 TC 8 Z9 8 U1 2 U2 21 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0020-7683 EI 1879-2146 J9 INT J SOLIDS STRUCT JI Int. J. Solids Struct. PD APR PY 2015 VL 58 BP 190 EP 200 DI 10.1016/j.ijsolstr.2015.01.001 PG 11 WC Mechanics SC Mechanics GA CD2RT UT WOS:000350927400016 ER PT J AU Ki, T Jeong, S AF Ki, Taekyung Jeong, Sangkwon TI Real-time measurement and analysis of energy flow in Stirling-type pulse tube refrigerator SO INTERNATIONAL JOURNAL OF THERMAL SCIENCES LA English DT Article DE Pulse tube refrigerator; Real-time measurement; Energy flow; Instantaneous measurement AB A stable instrument with the minimum void volume is developed for real-time measurement of physical conditions in Stirling-type pulse tube refrigerator. From the measured physical conditions, the energy flows are identified, so that we can precisely know the non-equilibrium energy conversion process in two Stirling-type pulse tube refrigerators. The results of this paper are the experimental results that are obtained from actual Stirling-type pulse tube refrigerator configurations. The proposed method can be useful for clarifying the energy conversion process and analyzing the tendency of physical conditions in cryogenic systems. (C) 2014 Elsevier Masson SAS. All rights reserved. C1 [Ki, Taekyung] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Engn, Magnet Dept, Berkeley, CA 94720 USA. [Jeong, Sangkwon] Korea Adv Inst Sci & Technol, Sch Mech Aerosp & Syst Engn, Div Mech Engn, Cryogen Engn Lab, Taejon 305701, South Korea. RP Ki, T (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Engn, Magnet Dept, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM tyki@lbl.gov; skjeong@kaist.ac.kr RI JEONG, SANGKWON/C-1547-2011 FU Space Core Technology Development Program of National Research Foundation of Korea - Ministry of Science, ICT & Future Planning (MSIP) [NRF-2013-042033] FX This research is supported by a grant from Space Core Technology Development Program of National Research Foundation of Korea (NRF-2013-042033) funded by Ministry of Science, ICT & Future Planning (MSIP). NR 14 TC 0 Z9 0 U1 0 U2 3 PU ELSEVIER FRANCE-EDITIONS SCIENTIFIQUES MEDICALES ELSEVIER PI PARIS PA 23 RUE LINOIS, 75724 PARIS, FRANCE SN 1290-0729 EI 1778-4166 J9 INT J THERM SCI JI Int. J. Therm. Sci. PD APR PY 2015 VL 90 BP 1 EP 8 DI 10.1016/j.ijthermalsci.2014.11.027 PG 8 WC Thermodynamics; Engineering, Mechanical SC Thermodynamics; Engineering GA CC1FV UT WOS:000350087500001 ER PT J AU Field, EK Sczyrba, A Lyman, AE Harris, CC Woyke, T Stepanauskas, R Emerson, D AF Field, Erin K. Sczyrba, Alexander Lyman, Audrey E. Harris, Christopher C. Woyke, Tanja Stepanauskas, Ramunas Emerson, David TI Genomic insights into the uncultivated marine Zetaproteobacteria at Loihi Seamount SO ISME JOURNAL LA English DT Article ID IRON-OXIDIZING ZETAPROTEOBACTERIA; PHOTOTROPHIC FE(II) OXIDATION; MULTIPLE SEQUENCE ALIGNMENT; SPECIES DEFINITION; ONE-CELL; BACTERIA; HAWAII; REDUCTION; OCEAN; PROTEOBACTERIA AB The Zetaproteobacteria are a candidate class of marine iron-oxidizing bacteria that are typically found in high iron environments such as hydrothermal vent sites. As much remains unknown about these organisms due to difficulties in cultivation, single-cell genomics was used to learn more about this elusive group at Loihi Seamount. Comparative genomics of 23 phylogenetically diverse single amplified genomes (SAGs) and two isolates indicate niche specialization among the Zetaproteobacteria may be largely due to oxygen tolerance and nitrogen transformation capabilities. Only Form II ribulose 1,5-bisphosphate carboxylase (RubisCO) genes were found in the SAGs, suggesting that some of the uncultivated Zetaproteobacteria may be adapted to low oxygen and/or high carbon dioxide concentrations. There is also genomic evidence of oxygen-tolerant cytochrome c oxidases and oxidative stress-related genes, indicating that others may be exposed to higher oxygen conditions. The Zetaproteobacteria also have the genomic potential for acquiring nitrogen from numerous sources including ammonium, nitrate, organic compounds, and nitrogen gas. Two types of molybdopterin oxidoreductase genes were found in the SAGs, indicating that those found in the isolates, thought to be involved in iron oxidation, are not consistent among all the Zetaproteobacteria. However, a novel cluster of redox-related genes was found to be conserved in 10 SAGs as well as in the isolates warranting further investigation. These results were used to isolate a novel iron-oxidizing Zetaproteobacteria. Physiological studies and genomic analysis of this isolate were able to support many of the findings from SAG analyses demonstrating the value of these data for designing future enrichment strategies. C1 [Field, Erin K.; Harris, Christopher C.; Stepanauskas, Ramunas; Emerson, David] Bigelow Lab Ocean Sci, East Boothbay, ME 04544 USA. [Sczyrba, Alexander] Univ Bielefeld, Ctr Biotechnol, D-33615 Bielefeld, Germany. [Lyman, Audrey E.] Colby Coll, Dept Biol, Waterville, ME 04901 USA. [Woyke, Tanja] US Dept Energy Joint Genome Inst, Walnut Creek, CA USA. RP Emerson, D (reprint author), Bigelow Lab Ocean Sci, 60 Bigelow Dr, East Boothbay, ME 04544 USA. EM demerson@bigelow.org OI Stepanauskas, Ramunas/0000-0003-4458-3108 FU NASA EPSCoR program administered through the Maine Space Consortium Grant [10-EPSCoR-0005]; National Science Foundation [OCE-0821374, OCE-1155754]; Office of Science of the US Department of Energy [DE-AC02-05CH11231]; Joint Genome Institute's Community Sequencing Program [560] FX We thank Brian Thompson, Nicole Poulton, and Elizabeth Fergusson for their technical expertise and support in single-cell sorting and sequencing, as well as Anna Leavitt for her assistance with the physiologic studies. We also thank the captains, crew and operators of the R/V Kilo Moana, R/V Thomas N Thompson, and Jason II ROV without whom this work would not have been possible. Last, we appreciate the intellectual input provided by the members of the Single Cell Genomics Center and Geomicrobiology labs at Bigelow. This work was financially supported by the NASA EPSCoR program administered through the Maine Space Consortium Grant 10-EPSCoR-0005 and the National Science Foundation Grants OCE-0821374 and OCE-1155754. The work conducted by the US Department of Energy Joint Genome Institute is supported by the Office of Science of the US Department of Energy under Contract No. DE-AC02-05CH11231. Additional sequencing support for Bigelow Laboratory was provided through the Joint Genome Institute's Community Sequencing Program, Project 560. NR 57 TC 10 Z9 10 U1 4 U2 15 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1751-7362 EI 1751-7370 J9 ISME J JI ISME J. PD APR PY 2015 VL 9 IS 4 BP 857 EP 870 DI 10.1038/ismej.2014.183 PG 14 WC Ecology; Microbiology SC Environmental Sciences & Ecology; Microbiology GA CD6NC UT WOS:000351204900007 PM 25303714 ER PT J AU Goltsman, DSA Comolli, LR Thomas, BC Banfield, JF AF Goltsman, Daniela S. Aliaga Comolli, Luis R. Thomas, Brian C. Banfield, Jillian F. TI Community transcriptomics reveals unexpected high microbial diversity in acidophilic biofilm communities SO ISME JOURNAL LA English DT Article ID RIBOSOMAL-RNA SEQUENCES; MAGNETOTACTIC BACTERIA; RIO TINTO; ECOLOGY; ACID; EVOLUTION; GENES; TOOLS; MINE; LIFE AB A fundamental question in microbial ecology relates to community structure, and how this varies across environment types. It is widely believed that some environments, such as those at very low pH, host simple communities based on the low number of taxa, possibly due to the extreme environmental conditions. However, most analyses of species richness have relied on methods that provide relatively low ribosomal RNA (rRNA) sampling depth. Here we used community transcriptomics to analyze the microbial diversity of natural acid mine drainage biofilms from the Richmond Mine at Iron Mountain, California. Our analyses target deep pools of rRNA gene transcripts recovered from both natural and laboratory-grown biofilms across varying developmental stages. In all, 91.8% of the similar to 254 million Illumina reads mapped to rRNA genes represented in the SILVA database. Up to 159 different taxa, including Bacteria, Archaea and Eukaryotes, were identified. Diversity measures, ordination and hierarchical clustering separate environmental from laboratory-grown biofilms. In part, this is due to the much larger number of rare members in the environmental biofilms. Although Leptospirillum bacteria generally dominate biofilms, we detect a wide variety of other Nitrospira organisms present at very low abundance. Bacteria from the Chloroflexi phylum were also detected. The results indicate that the primary characteristic that has enabled prior extensive cultivation-independent 'omic' analyses is not simplicity but rather the high dominance by a few taxa. We conclude that a much larger variety of organisms than previously thought have adapted to this extreme environment, although only few are selected for at any one time. C1 [Goltsman, Daniela S. Aliaga; Thomas, Brian C.; Banfield, Jillian F.] Univ Calif Berkeley, Environm Sci Policy & Management, Berkeley, CA 94720 USA. [Comolli, Luis R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Goltsman, DSA (reprint author), Univ Calif Berkeley, Environm Sci Policy & Management, 113 Hilgard Hall, Berkeley, CA 94720 USA. EM dgolts@eps.berkeley.edu; jbanfield@berkeley.edu FU NSF [1050680]; Department of Environmental Science, Policy, and Management at UC Berkeley; US Department of Energy, through the Carbon-Cycling program [DE-FG02-10ER64996]; Office of Science, Office of Basic Energy Sciences, of the US Department of Energy [DE-AC02-05CH11231] FX We thank the late Mr TW Arman, President, Iron Mountain Mines Inc., and Mr R Carver and M Jones for on-site assistance. We thank The Dimensions of Biodiversity Distributed Graduate Seminar (DBDGS, funded by NSF project 1050680) for useful discussions, Christopher Miller for providing purified RNA from the 4-way biofilm, and David Armitage for his help with diversity profiles R scripts. We thank the anonymous reviewers of this manuscript for their thoughtful and constructive comments. DSAG acknowledges funding from the Department of Environmental Science, Policy, and Management at UC Berkeley. This project was funded by the US Department of Energy, through the Carbon-Cycling (DE-FG02-10ER64996) program. LRC was supported by the Director, Office of Science, Office of Basic Energy Sciences, of the US Department of Energy under Contract No. DE-AC02-05CH11231. NR 55 TC 11 Z9 11 U1 9 U2 53 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1751-7362 EI 1751-7370 J9 ISME J JI ISME J. PD APR PY 2015 VL 9 IS 4 BP 1014 EP 1023 DI 10.1038/ismej.2014.200 PG 10 WC Ecology; Microbiology SC Environmental Sciences & Ecology; Microbiology GA CD6NC UT WOS:000351204900020 ER PT J AU Wang, YY Sun, X Wang, YD Zbib, HM AF Wang, Y. Y. Sun, X. Wang, Y. D. Zbib, H. M. TI Effects of Mn Content on the Deformation Behavior of Fe-Mn-Al-C TWIP Steels-A Computational Study SO JOURNAL OF ENGINEERING MATERIALS AND TECHNOLOGY-TRANSACTIONS OF THE ASME LA English DT Article DE stacking fault energy; Fe-Mn-Al-C TWIP steel; crystal plasticity finite element method; deformation twinning; boundary conditions ID STACKING-FAULT ENERGY; ALLOY AZ31; PLASTICITY; MECHANISM; TEXTURE; METALS; MODEL; DISLOCATIONS; DEPENDENCE; EVOLUTION AB This paper presents a double-slip/double-twin polycrystal plasticity model using finite element solution to investigate the kinetics of deformation twinning of medium manganese (Mn) twinning-induced plasticity (TWIP) steels. Empirical equations are employed to estimate the stacking fault energy (SFE) of TWIP steels and the critical resolved shear stress (CRSS) for dislocation slip and deformation twinning, respectively. The results suggest that the evolution of twinning in Fe-xMn-1.4Al-0.6C (x = 11.5, 13.5, 15.5, 17.5, and 19.5 mass%) TWIP steels, and its relation to the Mn content, can explain the effect of Mn on mechanical properties. By comparing the double-slip/double-twin model to a double-slip model, the predicted results essentially reveal that the interaction behavior between dislocation slip and deformation twinning can lead to an additional work hardening. Also, numerical simulations are carried out to study the influence of boundary conditions on deformation behavior and twin formation. The nucleation and growth of twinning are found to depend on internal properties (e.g., mismatch orientation of grains and stress redistribution) as well as on external constraints (e.g., the applied boundary conditions) of the material. C1 [Wang, Y. Y.; Wang, Y. D.] Northeastern Univ, Key Lab Anisotropy & Texture Mat, Shenyang 110819, Peoples R China. [Wang, Y. Y.; Sun, X.] Pacific NW Natl Lab, Computat Sci & Math Div, Richland, WA 99352 USA. [Wang, Y. D.] Univ Sci & Technol Beijing, State Key Lab Adv Met & Mat, Beijing 100083, Peoples R China. [Wang, Y. D.] Univ Sci & Technol Beijing, Collaborat Innovat Ctr Steel Technol, Beijing 100083, Peoples R China. [Zbib, H. M.] Washington State Univ, Sch Mech & Mat Engn, Pullman, WA 99164 USA. RP Sun, X (reprint author), Pacific NW Natl Lab, Computat Sci & Math Div, Richland, WA 99352 USA. EM xin.sun@pnnl.gov RI wang, yandong/G-9404-2013 FU U.S. Department of Energy (DOE) [DE-AC05-76RL01830]; DOE Office of Freedom CAR and Vehicle Technologies under the Automotive Lightweighting Materials Program; National Science Foundation of China [51231002]; Fundamental Research Funds for the Central Universities [06111020]; Qatar National Research Fund (a member of the Qatar Foundation) [NPRP 05-1294-2-559]; NPL [2012BA02] FX The Pacific Northwest National Laboratory is operated by the Battelle Memorial Institute for the U.S. Department of Energy (DOE) under Contract No. DE-AC05-76RL01830. This work was funded by the DOE Office of Freedom CAR and Vehicle Technologies under the Automotive Lightweighting Materials Program managed by. Mr. William Joost, National Science Foundation of China (Grant No. 51231002), and the Fundamental Research Funds for the Central Universities (Grant No. 06111020). H. M. Zbib acknowledges that his contribution to this publication was made possible by a National Priorities Research Program (Grant No. NPRP 05-1294-2-559) from the Qatar National Research Fund (a member of the Qatar Foundation). In addition, the support from NPL under Contract No. 2012BA02 is acknowledged. The statements made herein are the sole responsibility of the authors. NR 34 TC 0 Z9 0 U1 4 U2 33 PU ASME PI NEW YORK PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA SN 0094-4289 EI 1528-8889 J9 J ENG MATER-T ASME JI J. Eng. Mater. Technol.-Trans. ASME PD APR PY 2015 VL 137 IS 2 AR 021001 DI 10.1115/1.4029041 PG 9 WC Engineering, Mechanical; Materials Science, Multidisciplinary SC Engineering; Materials Science GA CD1BX UT WOS:000350809900001 ER PT J AU Valderrama, B Henderson, HB Gan, J Manuel, MV AF Valderrama, B. Henderson, H. B. Gan, J. Manuel, M. V. TI Influence of instrument conditions on the evaporation behavior of uranium dioxide with UV laser-assisted atom probe tomography SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID FIELD ION MICROSCOPE; FEMTOSECOND LASER; PULSED-LASER; NUCLEAR-FUEL; OPTIMIZATION; PERFORMANCE; OXIDE; UO2 AB Atom probe tomography (APT) provides the ability to detect subnanometer chemical variations spatially, with high accuracy. However, it is known that compositional accuracy can be affected by experimental conditions. A study of the effect of laser energy, specimen base temperature, and detection rate is performed on the evaporation behavior of uranium dioxide (UO2). In laser-assisted mode, tip geometry and standing voltage also contribute to the evaporation behavior. In this investigation, it was determined that modifying the detection rate and temperature did not affect the evaporation behavior as significantly as laser energy. It was also determined that three laser evaporation regimes are present in UO2. Very low laser energy produces a behavior similar to DC-field evaporation, moderate laser energy produces the desired laser-assisted field evaporation characteristic and high laser energy induces thermal effects, negatively altering the evaporation behavior. The need for UO2 to be analyzed under moderate laser energies to produce accurate stoichiometry distinguishes it from other oxides. The following experimental conditions providing the best combination of mass resolving power, accurate stoichiometry, and uniform evaporation behavior: 50 K, 10 pJ laser energy, a detection rate of 0.003 atoms per pulse, and a 100 kHz repetition rate. (C) 2015 Elsevier B.V. All rights reserved. C1 [Valderrama, B.; Henderson, H. B.; Manuel, M. V.] Univ Florida, Dept Mat Sci & Engn, Gainesville, FL 32611 USA. [Gan, J.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. RP Manuel, MV (reprint author), Univ Florida, 152 Rhines Hall, Gainesville, FL 32611 USA. EM mmanuel@mse.ufl.edu RI Manuel, Michele/A-8795-2009 OI Manuel, Michele/0000-0002-3495-7826 FU Center for Materials Science of Nuclear Fuel, Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [FWP 1356]; U.S. Department of Energy, Office of Nuclear Energy under DOE Idaho Operations Office [DE-AC07-051D14517] FX This paper is based on the work supported as part of the Center for Materials Science of Nuclear Fuel, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number FWP 1356. Use of the FIB and atom probe instrumentation at the Center for Advanced Energy Studies was supported by the U.S. Department of Energy, Office of Nuclear Energy under DOE Idaho Operations Office Contract DE-AC07-051D14517. The authors would also like to thank Dr. William Buyers for providing the UO2 sample used in this study and Dr. Yaqaio Wu for assistance in running the atom probe. NR 52 TC 1 Z9 1 U1 1 U2 8 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD APR PY 2015 VL 459 BP 37 EP 43 DI 10.1016/j.jnucmat.2014.12.119 PG 7 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA CC9SE UT WOS:000350710700006 ER PT J AU Xu, H Wu, L Zhu, J Navrotsky, A AF Xu, H. Wu, L. Zhu, J. Navrotsky, A. TI Synthesis, characterization and thermochemistry of Cs-, Rb- and Sr-substituted barium aluminium titanate hollandites SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID NUCLEAR-WASTE IMMOBILIZATION; SYNROC-TYPE HOLLANDITES; CESIUM SUBSTITUTION; RADIOACTIVE CESIUM; STRUCTURAL-ANALYSIS; SOLID-SOLUTIONS; PHASE; ENERGETICS; CHEMISTRY; DIFFRACTION AB Titanate hollandites are of considerable interest for immobilization of radioactive Cs, its daughter product Ba and related radionuclides Rb and Sr. In this study, we synthesized three hollandites, Ba1.18CS0.21Al2.44Ti5.53O16, Ba1.17Rb0.19Al2.46Ti5.53O16 and Ba1.4Sr0.10Al2.38Ti5.59O16, using sol-gel methods. Rietveld analysis of synchrotron XRD data shows that they adopt the tetragonal structure (space group I4/m), and their cell parameters increase with increasing cation size (Sr2+ --> Rb+ --> Cs+). Standard enthalpies of formation of these hollandites were determined from drop solution calorimetric measurements with lead borate as the solvent at 973 K. Their formation enthalpies are similar, consistent with the occurrence of extensive cation substitutions in hollandites. Further energetic analysis with respect to BaTiO3 and SrTiO3 perovskites and other oxides reveals decreased thermodynamic stability from Cs- to Rb- to Sr-hollandite. This trend is consistent with the phase assemblage observed in Synroc, where Cs+, Rb+ and Ba2+ enter into hollandite, whereas Sr2+ occurs in perovskite. (C) 2015 Elsevier B.V. All rights reserved. C1 [Xu, H.] Los Alamos Natl Lab, Earth & Environm Sci Div, Los Alamos, NM 87545 USA. [Wu, L.; Navrotsky, A.] Univ Calif Davis, Peter A Rock Thermochem Lab, Davis, CA 95616 USA. [Wu, L.; Navrotsky, A.] Univ Calif Davis, NEAT ORU, Davis, CA 95616 USA. [Zhu, J.] Los Alamos Natl Lab, Los Alamos Neutron Sci Ctr, Los Alamos, NM 87545 USA. RP Xu, H (reprint author), Los Alamos Natl Lab, Earth & Environm Sci Div, POB 1663, Los Alamos, NM 87545 USA. EM hxu@lanl.gov OI Xu, Hongwu/0000-0002-0793-6923 FU laboratory-directed research and development (LDRD) program of Los Alamos National Laboratory under DOE [DE-AC52-06NA25396]; U.S. DOE, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work was supported by the laboratory-directed research and development (LDRD) program of Los Alamos National Laboratory, which is operated by Los Alamos National Security LLC, under DOE Contract DE-AC52-06NA25396. Use of the Advanced Photon Source at Argonne National Laboratory was supported by the U.S. DOE, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 43 TC 4 Z9 4 U1 9 U2 42 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD APR PY 2015 VL 459 BP 70 EP 76 DI 10.1016/j.jnucmat.2015.01.014 PG 7 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA CC9SE UT WOS:000350710700010 ER PT J AU Perriot, R Liu, XY Stanek, CR Andersson, DA AF Perriot, R. Liu, X. -Y. Stanek, C. R. Andersson, D. A. TI Diffusion of Zr, Ru, Ce, Y, La, Sr and Ba fission products in UO2 SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; URANIUM-DIOXIDE; AB-INITIO; MOLECULAR-DYNAMICS; BASIS-SET; STABILITY; METALS; STATE; BEHAVIOR AB The diffusivity of the solid fission products (FP) Zr (Zr4+), Ru (Ru4+, Ru3+), Ce (Ce4+), Y (Y3+), La (La3+), Sr (Sr2+) and Ba (Ba2+) by a vacancy mechanism has been calculated, using a combination of density functional theory (DFT) and empirical potential (EP) calculations. The activation energies for the solid fission products are compared to the activation energy for Xe fission gas atoms calculated previously. Apart from Ru, the solid fission products all exhibit higher activation energy than Xe. For all solid FPs except y(3+), the migration of the FP has lower barrier than the migration of a neighboring U atom, making the latter the rate limiting step for direct migration. An indirect mechanism, consisting of two successive migrations around the FP, is also investigated. The calculated diffusivities show that most solid fission products diffuse with rates similar to U self-diffusion. However, Ru, Ba and Sr exhibit faster diffusion than the other solid FPs, with Ru3+ and Ru4+ diffusing even faster than Xe for T < 1200 K. The diffusivities correlate with the observed fission product solubility in UO2, and the tendency to form metallic and oxide second phase inclusions. (C) 2015 Elsevier B.V. All rights reserved. C1 [Perriot, R.; Liu, X. -Y.; Stanek, C. R.; Andersson, D. A.] Los Alamos Natl Lab, Mat Sci & Technol Div, Los Alamos, NM 87545 USA. RP Perriot, R (reprint author), Los Alamos Natl Lab, Mat Sci & Technol Div, POB 1663, Los Alamos, NM 87545 USA. EM rperriot@lanl.gov FU Department of Energy Nuclear Energy Advanced Modeling and Simulation (NEAMS) program FX This work was funded by the Department of Energy Nuclear Energy Advanced Modeling and Simulation (NEAMS) program. RP would like to thank Bias P. Uberuaga and Arthur F. Voter at LANL, for numerous discussions. NR 63 TC 5 Z9 5 U1 4 U2 35 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD APR PY 2015 VL 459 BP 90 EP 96 DI 10.1016/j.jnucmat.2015.01.001 PG 7 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA CC9SE UT WOS:000350710700013 ER PT J AU Bach, HT Anderoglu, O Saleh, TA Romero, TJ Kelsey, CT Olivas, ER Sencer, BH Dickerson, PO Connors, MA John, KD Maloy, SA AF Bach, H. T. Anderoglu, O. Saleh, T. A. Romero, T. J. Kelsey, C. T. Olivas, E. R. Sencer, B. H. Dickerson, P. O. Connors, M. A. John, K. D. Maloy, S. A. TI Proton irradiation damage of an annealed Alloy 718 beam window SO JOURNAL OF NUCLEAR MATERIALS LA English DT Review ID SPALLATION ENVIRONMENT; MECHANICAL-PROPERTIES; INCONEL-718 AB Mechanical testing and microstructural analysis was performed on an Alloy 718 window that was in use at the Los Alamos Neutron Science Center (LANSCE) Isotope Production Facility (IPF) for approximately 5 years. It was replaced as part of the IPF preventive maintenance program. The window was transported to the Wing 9 hot cells at the Chemical and Metallurgical Research (CMR) LANL facility, visually inspected and 3-mm diameter samples were trepanned from the window for mechanical testing and microstructural analysis. Shear punch testing and optical metallography was performed at the CMR hot cells. The 1-mm diameter shear punch disks were cut into smaller samples to further reduce radiation exposure dose rate using Focus Ion Beam (FIB) and microstructure changes were analyzed using a Transmission Electron Microscopy (TEM). Irradiation doses were determined to be similar to 0.2-0.7 dpa (edge) to 11.3 dpa (peak of beam intensity) using autoradiography and MCNPX calculations. The corresponding irradiation temperatures were calculated to be similar to 34-120 degrees C with short excursion to be similar to 47-220 degrees C using ANSYS. Mechanical properties and microstructure analysis results with respect to calculated dpa and temperatures show that significant work hardening occurs but useful ductility still remains. The hardening in the lowest dose region (similar to 0.2-0.7 dpa) was the highest and attributed to the formation of gamma '' precipitates and irradiation defect clusters/bubbles whereas the hardening in the highest dose region (similar to 11.3 dpa) was lower and attributed mainly to irradiation defect clusters and some thermal annealing. Published by Elsevier B.V. C1 [Bach, H. T.; Anderoglu, O.; Saleh, T. A.; Romero, T. J.; Kelsey, C. T.; Olivas, E. R.; Dickerson, P. O.; Connors, M. A.; John, K. D.; Maloy, S. A.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Sencer, B. H.] Idaho Natl Lab, Idaho Falls, ID 83402 USA. RP Bach, HT (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. RI Maloy, Stuart/A-8672-2009; OI Maloy, Stuart/0000-0001-8037-1319; John, Kevin/0000-0002-6181-9330; Olivas, Eric/0000-0002-7721-6622; Saleh, Tarik/0000-0003-2108-4293 FU U.S. Department of Energy, Office of Science, via Isotope Development and Production for Research and Applications subprogram in the Office of Nuclear Physics; Los Alamos National Laboratory (LANL)/Laboratory Directed Research & Development (LDRD) Program FX This material is based upon work supported by the U.S. Department of Energy, Office of Science, via funding from the Isotope Development and Production for Research and Applications subprogram in the Office of Nuclear Physics and the Los Alamos National Laboratory (LANL)/Laboratory Directed Research & Development (LDRD) Program. NR 16 TC 1 Z9 1 U1 3 U2 15 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD APR PY 2015 VL 459 BP 103 EP 113 DI 10.1016/j.jnucmat.2014.12.096 PG 11 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA CC9SE UT WOS:000350710700015 ER PT J AU Bailey, NA Stergar, E Toloczko, M Hosemann, P AF Bailey, Nathan A. Stergar, Erich Toloczko, Mychailo Hosemann, Peter TI Atom probe tomography analysis of high dose MA957 at selected irradiation temperatures SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID NANOSTRUCTURED FERRITIC ALLOYS; DISPERSION-STRENGTHENED STEELS; SPECIMEN PREPARATION; NEUTRON-IRRADIATION; MARTENSITIC STEELS; ODS STEELS; DEGREES-C; OXIDE; STABILITY; EVOLUTION AB Oxide dispersion strengthened CODS) alloys are meritable structural materials for nuclear reactor systems due to the exemplary resistance to radiation damage and high temperature creep. Summarized in this work are atom probe tomography (APT) investigations on a heat of MA957 that underwent irradiation in the form of in-reactor creep specimens in the Fast Flux Test Facility Materials Open Test Assembly (FFTF-MOTA) for the Liquid Metal Fast Breeder Reactor (LMFBR) program. The oxide precipitates appear stable under irradiation at elevated temperature over extended periods of time. Nominally, the precipitate chemistry is unchanged by the accumulated dose; although, evidence suggests that ballistic dissolution and reformation processes are occurring at all irradiation temperatures. At 412 degrees C-109 dpa, chromium enrichments - consistent with the alpha' phase - appear between the oxide precipitates, indicating radiation induced segregation. Grain boundaries, enriched with several elements including nickel and titanium, are observed at all irradiation conditions. At 412 degrees C-109 dpa, the grain boundaries are also enriched in molecular titanium oxide (TiO). (C) 2015 Elsevier B.V. All rights reserved. C1 [Bailey, Nathan A.; Stergar, Erich; Hosemann, Peter] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Stergar, Erich] CEN, SCK, BE-2400 Mol, Belgium. [Toloczko, Mychailo] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Hosemann, P (reprint author), Univ Calif Berkeley, 3117 Etcheverry Hall, Berkeley, CA 94720 USA. OI Hosemann, Peter/0000-0003-2281-2213 FU Nuclear Energy University Program (NEUP); NRC faculty development grant FX The authors would like to thank the ATR-NSUF user program for making the APT tool available to us. Fellowship funding was provided by the Nuclear Energy University Program (NEUP). Additional support was provided by the NRC faculty development grant. NR 60 TC 6 Z9 7 U1 4 U2 34 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD APR PY 2015 VL 459 BP 225 EP 234 DI 10.1016/j.jnucmat.2015.01.006 PG 10 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA CC9SE UT WOS:000350710700029 ER PT J AU Aitkaliyeva, A Madden, JW Miller, BD Cole, JI Gan, J AF Aitkaliyeva, Assel Madden, James W. Miller, Brandon D. Cole, James I. Gan, Jian TI Comparison of preparation techniques for nuclear materials for transmission electron microscopy (TEM) SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID FOCUSED ION-BEAM; GRAIN-GROWTH; IRRADIATION AB Preparation of highly radioactive and irradiated nuclear fuels and materials for transmission electron microscopy (TEM) is accompanied with a set of unique challenges. The paper evaluates three specimen preparation techniques for preparation of irradiated materials and determines which technique yields to the most reliable characterization of radiation damage microstructure. Various specimen preparation artifacts associated with each technique are considered and ways of minimizing these artifacts are addressed. Published by Elsevier B.V. C1 [Aitkaliyeva, Assel; Madden, James W.; Miller, Brandon D.; Cole, James I.; Gan, Jian] Idaho Natl Lab, Idaho Falls, ID 83415 USA. RP Aitkaliyeva, A (reprint author), Idaho Natl Lab, POB 1625,MS 6188, Idaho Falls, ID 83415 USA. EM assel.aitkaliyeva@inl.gov OI Aitkaliyeva, Assel/0000-0003-1481-6804 FU U.S. Department of Energy, under DOE Idaho Operations Office [DE-AC07-05ID14517] FX This work is supported by the U.S. Department of Energy, under DOE Idaho Operations Office Contract DE-AC07-05ID14517. Accordingly, the U.S. Government retains a nonexclusive, royalty-free license to publish or reproduce the published form of this contribution, or allow others to do so, for U.S. Government purposes. NR 16 TC 1 Z9 1 U1 2 U2 15 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD APR PY 2015 VL 459 BP 241 EP 246 DI 10.1016/j.jnucmat.2015.01.042 PG 6 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA CC9SE UT WOS:000350710700031 ER PT J AU Zhang, J Patel, MK Wang, YQ Tang, M Won, J Valdez, JA Sickafus, KE AF Zhang, J. Patel, M. K. Wang, Y. Q. Tang, M. Won, J. Valdez, J. A. Sickafus, K. E. TI Strong irradiation tolerance to amorphization in delta-Sc4Ti3O12 SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID RADIATION TOLERANCE; ION IRRADIATION; NUCLEAR-WASTE; PLUTONIUM; OXIDES; FUEL; IMMOBILIZATION; TRANSFORMATION; PYROCHLORES; DIFFRACTION AB Polycrystalline delta-phase Sc4Ti3O12 was irradiated under two separate conditions, with 200 key Ne+ or 600 keV Kr3+ at cryogenic temperature (similar to 77 K) to examine its radiation tolerance to amorphization. Irradiated samples were characterized using grazing incidence X-ray diffraction and cross-sectional transmission electron microscopy. An order-to-disorder (O-D) structural transformation was observed under both ion beam irradiation conditions, but the threshold irradiation doses to produce the O-D transformation differ significantly. The order to disorder phase transformation was completed by a fluence of 2 x 10(19) Ne/m(2) (or a peak dose of similar to 0.7 dpa) with Ne irradiation, while it was not accomplished until a fluence of 5 x 10(20) Kr/m(2) (or a peak dose of similar to 93 dpa) with Kr irradiation. This observation was interpreted in terms of greater probability of defect survivability in dilute Ne versus dense Kr ion cascades. More interesting aspect in this study, in the basis of so-called "chemical effects", Ti-bearing oxide Sc4Ti3O12 should be readily amorphous when exposed to ion irradiation, but no amorphization was observed even after 93 displacements per atom in Kr irradiation. These observations exhibit that the temperature-composition (T-C) phase diagram is a good indicator for radiation tolerance, especially for amorphization. (C) 2015 Elsevier B.V. All rights reserved. C1 [Zhang, J.] Xiamen Univ, Sch Energy, Xiamen 361005, Fujian, Peoples R China. [Zhang, J.; Wang, Y. Q.; Tang, M.; Won, J.; Valdez, J. A.; Sickafus, K. E.] Los Alamos Natl Lab, Mat Sci & Technol Div, Los Alamos, NM 87545 USA. [Patel, M. K.; Sickafus, K. E.] Univ Tennessee, Mat Sci & Engn Dept, Knoxville, TN 37996 USA. [Won, J.] Korea Basic Sci Inst, Div Electron Microscop Res, Taejon 305806, South Korea. RP Zhang, J (reprint author), Xiamen Univ, Sch Energy, Xiamen 361005, Fujian, Peoples R China. EM zhangjian@xmu.edu.cn OI won, Jonghan/0000-0002-7612-1322 FU US-DOE Office of Basic Energy Sciences (OBES), Division of Materials Sciences and Engineering; National Natural Science Foundation of China [11205128] FX This work was sponsored by US-DOE Office of Basic Energy Sciences (OBES), Division of Materials Sciences and Engineering. Partial support was provided to Zhang by the National Natural Science Foundation of China with Grant No. 11205128. NR 26 TC 0 Z9 0 U1 1 U2 12 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD APR PY 2015 VL 459 BP 265 EP 269 DI 10.1016/j.jnucmat.2015.01.057 PG 5 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA CC9SE UT WOS:000350710700034 ER PT J AU Neeway, JJ Abdelouas, A Ribet, S El Mendili, Y Schumacher, S Grambow, B AF Neeway, James J. Abdelouas, Abdesselam Ribet, Solange El Mendili, Yassine Schumacher, Stephan Grambow, Bernd TI Effect of Callovo-Oxfordian clay rock on the dissolution rate of the SON68 simulated nuclear waste glass SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID SECONDARY MINERAL PRECIPITATION; ALKALI FELDSPAR DISSOLUTION; 90 DEGREES-C; BOROSILICATE GLASS; BOOM-CLAY; RAMAN-SPECTROSCOPY; DIFFUSION; SILICA; RICH; TEMPERATURE AB Long-term storage of high-level nuclear waste glass in France is expected to occur in an engineered barrier system (EBS) located in a subsurface Callovo-Oxfordian (COx) clay rock formation in the Paris Basin in northeastern France. Understanding the behavior of glass dissolution in the complex system is critical to be able to reliably model the performance of the glass in this complex environment. To simulate this multi-barrier repository scenario in the laboratory, several tests have been performed to measure glass dissolution rates of the simulated high-level nuclear waste glass, SON68, in the presence of COx claystone at 90 degrees C. Experiments utilized a High-Performance Liquid Chromatography (HPLC) pump to pass simulated Bure site COx pore water through a reaction cell containing SON68 placed between two COx claystone cores for durations up to 200 days. Silicon concentrations at the outlet were similar in all experiments, even the blank experiment with only the COx claystone (similar to 4 mg/L at 25 degrees C and similar to 15 mg/L at 90 degrees C). The steady-state pH of the effluent, measured at room temperature, was roughly 7.1 for the blank and 7.3-7.6 for the glass-containing experiments demonstrating the pH buffering capacity of the COx claystone. Dissolution rates for SON68 in the presence of the claystone were elevated compared to those obtained from flow-through experiments conducted with SON68 without claystone in silica-saturated solutions at the same temperature and similar pH values. Additionally, through surface examination of the monoliths, the side of the monolith in direct contact with the claystone was seen to have a corrosion thickness 2.5 x greater than the side in contact with the bulk glass powder. Results from one experiment containing Si-32-doped SON68 also suggest that the movement of Si through the claystone is controlled by a chemically coupled transport with a Si retention factor, K-d, of 900 mL/g. (C) 2015 Elsevier B.V. All rights reserved. C1 [Neeway, James J.; Abdelouas, Abdesselam; Ribet, Solange; El Mendili, Yassine; Grambow, Bernd] Univ Nantes, SUBATECH, UMR 6457, Ecole Mines Nantes,CNRS,IN2P3, F-44307 Nantes 3, France. [Schumacher, Stephan] ANDRA, F-92298 Chatenay Malabry, France. RP Neeway, JJ (reprint author), Pacific NW Natl Lab, POB 999, Richland, WA 99354 USA. EM James.Neeway@pnnl.gov OI Neeway, Jim/0000-0001-7046-8408 NR 60 TC 2 Z9 2 U1 5 U2 22 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD APR PY 2015 VL 459 BP 291 EP 300 DI 10.1016/j.jnucmat.2015.01.054 PG 10 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA CC9SE UT WOS:000350710700038 ER PT J AU Riley, BJ Pierce, DA Frank, SM Matyas, J Burns, CA AF Riley, Brian J. Pierce, David A. Frank, Steven M. Matyas, Josef Burns, Carolyne A. TI Efficacy of a solution-based approach for making sodalite waste forms for an oxide reduction salt utilized in the reprocessing of used uranium oxide fuel SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID SOL-GEL TRANSITION; ELECTROCHEMICAL REDUCTION; NEUTRON-DIFFRACTION; HALIDE SODALITES; SIMPLE SILICATES; STATE NMR; GLASS; LICL; UO2 AB This paper describes the various approaches evaluated for making solution-derived sodalite with a LiCl-Li2O oxide reduction salt selected to dissolve used uranium oxide fuel so the uranium can be recovered and recycled. The approaches include modified sol-gel and solution-based synthesis processes. As-made products were mixed with 5 and 10 mass% of a Na2O-B2O3-SiO2 glass binder and these, along with product without a binder, were heated using either a cold-press-and-sinter method or hot uniaxial pressing. The results demonstrate the limitation of sodalite yield due to the fast intermediate reactions between Na+ and Cl- to form halite in solution and Li2O and SiO2 to form lithium silicates (e.g., Li2SiO3 or Li2Si2O5) in the calcined and sintered pellets. The results show that pellets can be made with high sodalite fractions in the crystalline product (similar to 92 mass%) and low porosities using a solution-based approach and this LiCl-Li2O salt but that the incorporation of Li into the sodalite is low. (C) 2014 Elsevier B.V. All rights reserved. C1 [Riley, Brian J.; Pierce, David A.; Matyas, Josef; Burns, Carolyne A.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Frank, Steven M.] Idaho Natl Lab, Idaho Falls, ID 83402 USA. RP Riley, BJ (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM brian.riley@pnnl.gov RI Frank, Steven/B-9046-2017; OI Frank, Steven/0000-0001-8259-6722; Riley, Brian/0000-0002-7745-6730 FU U.S. Department of Energy Office of Nuclear Energy Joint Fuel Cycle Studies; [DE-AC05-76RL01830]; [DE-AC07-05ID14517] FX The Pacific Northwest National Laboratory is operated by Battelle under Contract Number DE-AC05-76RL01830 and the Idaho National Laboratory is operated under contract DE-AC07-05ID14517. The authors would also like to express thanks to the U.S. Department of Energy Office of Nuclear Energy Joint Fuel Cycle Studies staff and leadership that funded and provided oversight to this work that include K. Bateman, K. Marsden, and M. Goff. Authors would also like to express thanks for assistance from X. Li for help with BET measurements; J. McCloy, J. Crum, and J. Westsik for helpful comments on the manuscript; and C. Chamberlin and S. Carlson for help with cutting and polishing specimens. NR 47 TC 1 Z9 1 U1 5 U2 15 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD APR PY 2015 VL 459 BP 313 EP 322 DI 10.1016/j.jnucmat.2014.09.042 PG 10 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA CC9SE UT WOS:000350710700041 ER PT J AU Matlack, KH Bradley, HA Thiele, S Kim, JY Wall, JJ Jung, HJ Qu, JM Jacobs, LJ AF Matlack, Kathryn H. Bradley, Harrison A. Thiele, Sebastian Kim, Jin-Yeon Wall, James J. Jung, Hee Joon Qu, Jianmin Jacobs, Laurence J. TI Nonlinear ultrasonic characterization of precipitation in 17-4PH stainless steel SO NDT & E INTERNATIONAL LA English DT Article DE Nonlinear ultrasonic methods; Thermal embrittlement; Precipitate hardening; Nonlinear Rayleigh waves ID RAYLEIGH SURFACE-WAVES; HARMONIC-GENERATION; RPV STEELS; MICROSTRUCTURAL EVOLUTION; MODEL ALLOYS; EMBRITTLEMENT; KINETICS; DAMAGE; PERSPECTIVE; FE AB This research is part of a broader effort to develop a nondestructive evaluation technique to monitor radiation damage in reactor pressure vessel steels, the main contributor being copper-rich precipitates. In this work, 17-4PH stainless steel is thermally aged to study the effects of copper precipitates on the acoustic nonlinearity parameter. Nonlinear ultrasonic measurements using Rayleigh waves are performed on isothermally aged 17-4PH. Results showed a decrease in the acoustic nonlinearity parameter with increasing aging time, consistent with evidence of copper precipitation from hardness, thermoelectric power, transmission electron microscopy, and atom probe tomography measurements. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Matlack, Kathryn H.] Swiss Fed Inst Technol, Dept Mech & Proc Engn, CH-8092 Zurich, Switzerland. [Bradley, Harrison A.; Wall, James J.; Jacobs, Laurence J.] Georgia Inst Technol, GW Woodruff Sch Mech Engn, Atlanta, GA 30332 USA. [Thiele, Sebastian; Kim, Jin-Yeon; Jacobs, Laurence J.] Georgia Inst Technol, Sch Civil & Environm Engn, Atlanta, GA 30332 USA. [Wall, James J.] Elect Power Res Inst, Charlotte, NC 28262 USA. [Jung, Hee Joon] Pacific NW Natl Lab, Richland, WA 99354 USA. [Qu, Jianmin] Northwestern Univ, Dept Civil & Environm Engn, Evanston, IL 60208 USA. RP Matlack, KH (reprint author), Swiss Fed Inst Technol, Dept Mech & Proc Engn, CH-8092 Zurich, Switzerland. EM matlackk@ethz.ch RI Qu, Jianmin/E-3521-2010; Kim, Jin-Yeon/C-2179-2008; OI Kim, Jin-Yeon/0000-0002-5518-0032; Matlack, Kathryn/0000-0001-7387-2414; Jacobs, Laurence/0000-0002-0358-7973 FU Office of Biological and Environmental Research; DOE Office of Nuclear Energy's Nuclear Energy University Programs (NEUP) FX A portion of this research was performed using EMSL, a DOE Office of Science User Facility sponsored by the Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. The authors would like to thank Dan Edwards and Alicia Certain at Pacific Northwest National Laboratory for their help with the TEM and APT measurements and interpretations. This research is being performed using funding received from the DOE Office of Nuclear Energy's Nuclear Energy University Programs (NEUP). NR 38 TC 7 Z9 7 U1 5 U2 24 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0963-8695 EI 1879-1174 J9 NDT&E INT JI NDT E Int. PD APR PY 2015 VL 71 BP 8 EP 15 DI 10.1016/j.ndteint.2014.11.001 PG 8 WC Materials Science, Characterization & Testing SC Materials Science GA CD0RV UT WOS:000350782500002 ER PT J AU Weldon, RA Fensin, ML Trellue, HR AF Weldon, R. A., Jr. Fensin, M. L. Trellue, H. R. TI Total neutron emission generation and characterization for a Next Generation Safeguards Initiative spent fuel library SO PROGRESS IN NUCLEAR ENERGY LA English DT Article DE Total neutron emission; Spent fuel characterization; NGSI; MCNP AB In March of 2009 the Next Generation Safeguards Initiative of the U.S. Department of Energy began a nominal five year spent fuel research effort with the goal of: (1) quantifying plutonium content in spent nuclear fuel through the use of non-destructive assay (NDA) techniques; (2) quantifying the capability of these NDA techniques to quantify burnup, cooling time, and initial enrichment, as well as detect pin diversions, for spent fuel assemblies. These NDA techniques were first scoped in computation space in order to understand detection limitations and down select for further testing. Multiple Monte Carlo based spent fuel libraries (SFL's) were developed to be used as source terms for assessing the detection limitations of each of these techniques. The characterization of the SFL's provide an analysis of different burn strategies used for spent fuel, functional fits for state point analysis, and the components of the neutron signal. This paper details both a methodology for generating the spatially dependent gross neutron emission (GNE) as well as a characterization of the GNE for a particular NGSI SFL for two different shuffle patterns. The GNE was characterized by examining three major components: (1) the total neutron emission; (2) the (alpha, n) and spontaneous fission emissions; and (3) the main contributors to the spontaneous fission and (alpha, n) emission signals. The total neutron emission was characterized by looking at two different shuffle patterns and using three different pin analysis techniques. The pin analysis techniques used were: (1) sum all the pins in the assembly; (2) create four pin zones to be summed; and (3) examine specific pins. These characterizations provide a large set of data with integral values (cooling time vs emission and burnup vs emission) and derivative values (isotopic percent composition) with visual depiction and detailed explanation. The characterizations also provide a comparison of the effects of shuffle schemes on the neutron emission signal for two different shuffle patterns. This data can be used in the development of time and burnup dependent normalized functions to describe the trends displayed in the data. This study also shows that the information which can be obtained from the GNE depends upon how the information is grouped and analyzed. Summing all the pins of the assembly or assuming a uniform burnup results in the loss of valuable neutron emission information. By splitting the pins into zones, trends such as the total emissions across the assembly become evident. By evaluating individual pins trends such as the effect of water rods on the neutron emission become evident. This type of analysis can be of great use to safeguards. Evaluating the GNE on a pin by pin basis leads to a much clearer picture of the constituents of the assembly. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Weldon, R. A., Jr.; Fensin, M. L.; Trellue, H. R.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Weldon, RA (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA. FU Next Generation Safeguards Initiative (NGSI), Office of Nonproliferation and International Security (NIS), National Nuclear Security Administration (NNSA) FX The authors would like to acknowledge the support of the Next Generation Safeguards Initiative (NGSI), Office of Nonproliferation and International Security (NIS), National Nuclear Security Administration (NNSA). NR 19 TC 0 Z9 0 U1 0 U2 2 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0149-1970 J9 PROG NUCL ENERG JI Prog. Nucl. Energy PD APR PY 2015 VL 80 BP 45 EP 73 DI 10.1016/j.pnucene.2014.10.012 PG 29 WC Nuclear Science & Technology SC Nuclear Science & Technology GA CD0QR UT WOS:000350779500006 ER PT J AU Gao, M Guttikunda, SK Carmichael, GR Wang, YS Liu, ZR Stanier, CO Saide, PE Yu, M AF Gao, Meng Guttikunda, Sarath K. Carmichael, Gregory R. Wang, Yuesi Liu, Zirui Stanier, Charles O. Saide, Pablo E. Yu, Man TI Health impacts and economic losses assessment of the 2013 severe haze event in Beijing area SO SCIENCE OF THE TOTAL ENVIRONMENT LA English DT Article DE Haze; PM2.5; Beijing; WRF-Chem; Health impacts; Economic losses ID PARTICULATE AIR-POLLUTION; CHINESE CITIES; GLOBAL BURDEN; URBAN AREAS; EXPOSURE; DISEASE; PM2.5; MODEL; PM10; FOG AB Haze is a serious air pollution problem in China, especially in Beijing and surrounding areas, affecting visibility, public health and regional climate. In this study, the Weather Research and Forecasting-Chemistry (WRF-Chem) model was used to simulate PM2.5 (particulate matters with aerodynamic diameter <= 2.5 mu m) concentrations during the 2013 severe haze event in Beijing, and health impacts and health-related economic losses were calculated based on model results. Compared with surface monitoring data, the model results reflected pollution concentrations accurately (correlation coefficients between simulated and measured PM2.5 were 0.7, 0.4, 0.5 and 0.6 in Beijing, Tianjin, Xianghe and Xinglong stations, respectively). Health impacts assessments show that the PM2.5 concentrations in January might cause 690 (95% confidence interval (CI): (490, 890)) premature deaths, 45,350(95% CI: (21,640, 57,860)) acute bronchitis and 23,720 (95% Cl: (17,090, 29,710)) asthma cases in Beijing area. Results of the economic losses assessments suggest that the haze in January 2013 might lead to 253.8 (95% CI: (170.2, 331.2)) million US$ losses, accounting for 0.08% (95% CI: (0.05%, 0.1%)) of the total 2013 annual gross domestic product (GDP) of Beijing. (C) 2015 Elsevier B.V. All rights reserved. C1 [Gao, Meng; Carmichael, Gregory R.; Stanier, Charles O.; Saide, Pablo E.; Yu, Man] Univ Iowa, Ctr Global & Reg Environm Res, Iowa City, IA 52242 USA. [Guttikunda, Sarath K.] Desert Res Inst, Div Atmospher Sci, Reno, NV 89512 USA. [Wang, Yuesi; Liu, Zirui] Chinese Acad Sci, Inst Atmospher Phys, State Key Lab Atmospher Boundary Layer Phys & Atm, Beijing 100029, Peoples R China. [Yu, Man] Argonne Natl Lab, Math & Comp Sci Div, Argonne, IL 60439 USA. RP Gao, M (reprint author), Univ Iowa, Ctr Global & Reg Environm Res, Iowa City, IA 52242 USA. EM meng-gao@uiowa.edu RI Stanier, Charles/D-4307-2016; Gao, Meng/P-8921-2015 OI Stanier, Charles/0000-0001-9924-0853; Gao, Meng/0000-0002-8657-3541 FU NIEHS NIH HHS [P30 ES005605] NR 42 TC 30 Z9 32 U1 16 U2 184 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0048-9697 EI 1879-1026 J9 SCI TOTAL ENVIRON JI Sci. Total Environ. PD APR 1 PY 2015 VL 511 BP 553 EP 561 DI 10.1016/j.scitotenv.2015.01.005 PG 9 WC Environmental Sciences SC Environmental Sciences & Ecology GA CC6YC UT WOS:000350513900059 PM 25585158 ER PT J AU Cohen, ML AF Cohen, Marvin L. TI Superconductivity in modified semiconductors and the path to higher transition temperatures SO SUPERCONDUCTOR SCIENCE & TECHNOLOGY LA English DT Review DE superconductivity; semi conductors; low temperature ID NORM-CONSERVING PSEUDOPOTENTIALS; STRONG-COUPLED SUPERCONDUCTORS; ELECTRON-PHONON INTERACTIONS; CARBON NANOTUBES; TOTAL-ENERGY; SI; MOMENTUM; DIAMOND; SOLIDS; SYSTEM AB After some background discussion on experimental, theoretical, and computational developments in superconductivity, this review will focus on some areas of theoretical studies of superconductivity in semiconductor or insulating materials that have been modified to have carriers at low temperatures. The possible path to higher superconducting transition temperatures will also be discussed using some of what was learned from the study of semiconductor systems. C1 [Cohen, Marvin L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Phys, Berkeley, CA 94720 USA. [Cohen, Marvin L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Cohen, ML (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Phys, Berkeley, CA 94720 USA. EM mlcohen@berkeley.edu FU National Science Foundation [DMR10-1006184]; Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division of the US Department of Energy [DE-AC02-05CH11231] FX This work was supported by the National Science Foundation Grant No DMR10-1006184 and Director, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division of the US Department of Energy under Contract No. DE-AC02-05CH11231. NR 68 TC 1 Z9 1 U1 5 U2 39 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-2048 EI 1361-6668 J9 SUPERCOND SCI TECH JI Supercond. Sci. Technol. PD APR PY 2015 VL 28 IS 4 AR 043001 DI 10.1088/0953-2048/28/4/043001 PG 8 WC Physics, Applied; Physics, Condensed Matter SC Physics GA CD4LY UT WOS:000351055500002 ER PT J AU Her, JL Kohama, Y Matsuda, YH Kindo, K Yang, WH Chareev, DA Mitrofanova, ES Volkova, OS Vasiliev, AN Lin, JY AF Her, J. L. Kohama, Y. Matsuda, Y. H. Kindo, K. Yang, W-H Chareev, D. A. Mitrofanova, E. S. Volkova, O. S. Vasiliev, A. N. Lin, J-Y TI Anisotropy in the upper critical field of FeSe and FeSe0.33Te0.67 single crystals SO SUPERCONDUCTOR SCIENCE & TECHNOLOGY LA English DT Article DE superconductivity phase diagrams; transition temperature variations; phase diagrams; pnictides and chalcogenides ID CRITICAL MAGNETIC-FIELD; SUPERCONDUCTIVITY; TEMPERATURE; DEPENDENCE AB The electric resistivity of single crystalline Fe-based superconductors FeSe and FeSe0.33Te0.67 was measured in pulsed magnetic fields up to 55 T. Te-doped iron selenide, FeSe0.33Te0.67, shows rather isotropic behavior in both magnetoresistance (MR) and upper critical fields (H-c2(perpendicular to)(0)/H-c2(parallel to)(0) = 48 T/42 T similar to 1.14), when an external magnetic field is applied parallel and perpendicular to the crystallographic c-axis. These isotropic behaviors are frequently observed in an iron-based superconductor, and the isotropy in H-c2 can likely be described by the Pauli effect. In contrast, our measurements elucidate that the undoped iron selenide, FeSe, exhibits a clear anisotropy in both MR and H-c2 (H-c2(perpendicular to)(0)/H-c2(parallel to)(0) = 27 T/15 T similar to 1.8). This behavior occurs because the clean in-plane conduction (RRR = 35) allows to form a closed electron orbit within the two-dimensional Fermi sheets only for the magnetic field parallel to the c-axis, which results in an appearance of an intrinsic (orbital-effect limited) upper critical field for the undoped FeSe. Doping of Te breaks the clean in-plane conduction and leads to a crossover from an orbital limit dominating behavior to a Pauli limit dominating one. C1 [Her, J. L.] Chang Gung Univ, Div Nat Sci, Ctr Gen Educ, Taoyuan 333, Taiwan. [Kohama, Y.; Matsuda, Y. H.; Kindo, K.] Univ Tokyo, Inst Solid State Phys, Kashiwa, Chiba 2778581, Japan. [Yang, W-H; Lin, J-Y] Natl Chiao Tung Univ, Inst Phys, Hsinchu 30010, Taiwan. [Chareev, D. A.] Russian Acad Sci, Inst Expt Mineral, Chernogolovka 142432, Russia. [Mitrofanova, E. S.; Volkova, O. S.; Vasiliev, A. N.] Moscow MV Lomonosov State Univ, Dept Low Temp Phys & Superconduct, Fac Phys, Moscow 119991, Russia. [Volkova, O. S.; Vasiliev, A. N.] Ural Fed Univ, Theoret Phys & Appl Math Dept, Ekaterinburg 620002, Russia. [Vasiliev, A. N.] Natl Univ Sci & Technol MISiS, Moscow 119049, Russia. [Lin, J-Y] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Her, JL (reprint author), Chang Gung Univ, Div Nat Sci, Ctr Gen Educ, Taoyuan 333, Taiwan. EM her@mail.cgu.edu.tw RI Volkova, Olga/A-4072-2008; Chareev, Dmitriy/B-8504-2009; Mitrofanova, Ekaterina/E-2942-2015; Vasiliev, Alexander/A-7562-2008 OI Chareev, Dmitriy/0000-0002-9380-2680; FU National Science Council of Taiwan [NSC101-2112-M-182-001-MY3, NSC-101-2112-M-009-017-MY2]; MOE ATU program at NCTU; Russian Foundation for Basic Research [14-02-92002]; Civilian Research and Development Foundation [FSAX-14-60108-0]; RF [MK-7138.2013.2]; JSPS [25800187]; Ministry of Education and Science of the Russian Federation in the framework of Increase Competitiveness Program of NUST "MISiS" [K2-2014-036] FX This work was supported by National Science Council of Taiwan under Grant Nos. NSC101-2112-M-182-001-MY3, NSC-101-2112-M-009-017-MY2, the MOE ATU program at NCTU, Russian Foundation for Basic Research under Grant 14-02-92002, and Civilian Research and Development Foundation under Grant FSAX-14-60108-0. JYL would like to thank ALS for support. OSV acknowledges support of RF President Grant MK-7138.2013.2. YK was supported by JSPS Grant-in-Aid Young Scientists (B) 25800187. This work was supported in part from the Ministry of Education and Science of the Russian Federation in the framework of Increase Competitiveness Program of NUST "MISiS" (No. K2-2014-036). NR 29 TC 8 Z9 8 U1 6 U2 48 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-2048 EI 1361-6668 J9 SUPERCOND SCI TECH JI Supercond. Sci. Technol. PD APR PY 2015 VL 28 IS 4 AR 045013 DI 10.1088/0953-2048/28/4/045013 PG 6 WC Physics, Applied; Physics, Condensed Matter SC Physics GA CD4LY UT WOS:000351055500019 ER PT J AU Mitchell, JE Hillesheim, DA Bridges, CA Paranthaman, MP Gofryk, K Rindfleisch, M Tomsic, M Sefat, AS AF Mitchell, Jonathan E. Hillesheim, Daniel A. Bridges, Craig A. Paranthaman, M. Parans Gofryk, Kris Rindfleisch, Matt Tomsic, Mike Sefat, Athena S. TI Optimization of a non-arsenic iron-based superconductor for wire fabrication SO SUPERCONDUCTOR SCIENCE & TECHNOLOGY LA English DT Article DE iron based superconductor; selenide wire; non arsenic ID CRITICAL-CURRENT DENSITY; CRITICAL FIELD HC2; PURITY DEPENDENCE; TEMPERATURE; TAPES AB We report on the optimization of synthesis of iron selenide-based superconducting powders and the fabrication of selenide-based wire. The powders were synthesized by an ammonothermal method, whereby Ba is intercalated between FeSe layers to produce Ba-x(NH3)(y)Fe2Se2, with tetragonal structure similar to AFe(2)X(2) (X: As, Se), '122', superconductors. The optimal T-c (up to 38 K) and Meissner and shielding superconducting fractions are obtained from the shortest reaction time (t) of reactants in liquid ammonia (30 min). With the increase of t, a second crystalline 122 phase, with a smaller unit cell, emerges. A small amount of NH3 is released from the structure above similar to 200 degrees C, which results in loss of superconductivity. However, in the confined space of niobium/Monel tubing, results indicate there is enough pressure for some of NH3 to remain in the crystal lattice, and thermal annealing can be performed at temperatures of up to 780 degrees C, increasing wire density and yielded a reasonable T-c approximate to 16 K. Here, we report of the first successful wire fabrication of non-arsenic high-T-c iron-based superconductor. Although bulk materials are estimated to carry critical current densities > 100 kA cm(-2) (4 K, self-field), the current transport within wires need to be optimized (J(c) similar to 1 kA cm(-2)). C1 [Mitchell, Jonathan E.; Gofryk, Kris; Sefat, Athena S.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Hillesheim, Daniel A.; Bridges, Craig A.; Paranthaman, M. Parans] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Rindfleisch, Matt; Tomsic, Mike] Hyper Tech Res Inc, Columbus, OH 43228 USA. RP Mitchell, JE (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. EM sefata@ornl.gov RI Paranthaman, Mariappan/N-3866-2015; Sefat, Athena/R-5457-2016; OI Paranthaman, Mariappan/0000-0003-3009-8531; Sefat, Athena/0000-0002-5596-3504; Gofryk, Krzysztof/0000-0002-8681-6857 FU Oak Ridge National Laboratory (ORNL) SEED funding program; US Department of Energy, Office of Science, Office of Basic Energy Sciences, Materials Science and Engineering Division FX Iron-based superconductor wire fabrication research was supported by the Oak Ridge National Laboratory (ORNL) SEED funding program. AS also acknowledges support by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, Materials Science and Engineering Division, for some of the powder synthesis efforts. The team acknowledges C Cantoni for group discussions, and also specifically for tube filling, wire cutting, and keeping annealing-temperature records of wires. NR 43 TC 2 Z9 2 U1 2 U2 20 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-2048 EI 1361-6668 J9 SUPERCOND SCI TECH JI Supercond. Sci. Technol. PD APR PY 2015 VL 28 IS 4 AR 045018 DI 10.1088/0953-2048/28/4/045018 PG 8 WC Physics, Applied; Physics, Condensed Matter SC Physics GA CD4LY UT WOS:000351055500024 ER PT J AU Dong, AY Fu, Q Wei, MM Liu, Y Ning, YX Yang, F Bluhm, H Bao, XH AF Dong, Aiyi Fu, Qiang Wei, Mingming Liu, Yun Ning, Yanxiao Yang, Fan Bluhm, Hendrik Bao, Xinhe TI Facile oxygen intercalation between full layer graphene and Ru(0001) under ambient conditions SO SURFACE SCIENCE LA English DT Article DE Graphene; Intercalation; AP-XPS; Oxidation; Ru(0001) ID SCANNING-TUNNELING-MICROSCOPY; EPITAXIAL GRAPHENE; METAL-SURFACES; OXIDATION; MONOLAYER; GRAPHITE; GROWTH; CO; DECOMPOSITION; SPECTROSCOPY AB Graphene coatings have been widely considered as protection layers on metal surfaces to prevent surface oxidation and corrosion in gaseous atmospheres. Here, using in-situ ambient pressure X-ray photoelectron spectroscopy we demonstrate that oxygen intercalation readily occurs at full monolayer graphene/Ru(0001) interfaces in 0.5 Torr O-2 around 150 degrees C, resulting in decoupling of the graphene overlayer from the Ru surface and oxidation of the metal surface. Moreover, oxygen intercalation has been observed even upon illumination of the graphene/Ru(0001) surface with an infrared lamp in air. These results indicate that the stability of graphene/metal interfaces under ambient conditions should be taken into consideration for future applications. (C) 2014 Elsevier B.V. All rights reserved. C1 [Dong, Aiyi; Fu, Qiang; Wei, Mingming; Liu, Yun; Ning, Yanxiao; Yang, Fan; Bao, Xinhe] Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China. [Bluhm, Hendrik] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Fu, Q (reprint author), Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China. EM qfu@dicp.ac.cn RI Fu, Qiang/E-7109-2015; YANG, FAN/J-2706-2012 OI Fu, Qiang/0000-0001-5316-6758; YANG, FAN/0000-0002-1406-9717 FU National Natural Science Foundation of China [21222305, 21373208, 21033009]; Ministry of Science and Technology of China [2011CB932704, 2013CB834603]; Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences and Materials Sciences Division of the US Department of Energy at the Lawrence Berkeley National Laboratory [DE-AC02-05CH11231] FX This work was financially supported by the National Natural Science Foundation of China (No. 21222305, No. 21373208, and No. 21033009), and Ministry of Science and Technology of China (No. 2011CB932704 and No. 2013CB834603). The ALS and the MES beamline 11.0.2 are supported by the Director, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences and Materials Sciences Division of the US Department of Energy at the Lawrence Berkeley National Laboratory under Contract No. DE-AC02-05CH11231. NR 53 TC 14 Z9 14 U1 4 U2 55 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0039-6028 EI 1879-2758 J9 SURF SCI JI Surf. Sci. PD APR PY 2015 VL 634 SI SI BP 37 EP 43 DI 10.1016/j.susc.2014.10.008 PG 7 WC Chemistry, Physical; Physics, Condensed Matter SC Chemistry; Physics GA CC1HO UT WOS:000350092000007 ER PT J AU Rogers, DM Kent, MS Rempe, SB AF Rogers, David M. Kent, Michael S. Rempe, Susan B. TI Molecular basis of endosomal-membrane association for the dengue virus envelope protein SO BIOCHIMICA ET BIOPHYSICA ACTA-BIOMEMBRANES LA English DT Article DE Fusion; Free energy; Multi-scale models; Membrane bending ID BORNE ENCEPHALITIS-VIRUS; SEMLIKI-FOREST-VIRUS; HUMAN DENDRITIC CELLS; LIPID-BILAYERS; FORCE-FIELD; CONFORMATIONAL-CHANGES; DYNAMICS SIMULATIONS; HEPARAN-SULFATE; FUSION PROTEIN; STALK MODEL AB Dengue virus is coated by an icosahedral shell of 90 envelope protein dimers that convert to trimers at low pH and promote fusion of its membrane with the membrane of the host endosome. We provide the first estimates for the free energy barrier and minimum for two key steps in this process: host membrane bending and protein-membrane binding. Both are studied using complementary membrane elastic, continuum electrostatics and all-atom molecular dynamics simulations. The predicted host membrane bending required to form an initial fusion stalk presents a 22-30 kcal/mol free energy barrier according to a constrained membrane elastic model. Combined continuum and molecular dynamics results predict a 15 kcal/mol free energy decrease on binding of each trimer of dengue envelope protein to a membrane with 30% anionic phosphatidylglycerol lipid. The bending cost depends on the preferred curvature of the lipids composing the host membrane leaflets, while the free energy gained for protein binding depends on the surface charge density of the host membrane. The fusion loop of the envelope protein inserts exactly at the level of the interface between the membrane's hydrophobic and head-group regions. The methods used in this work provide a means for further characterization of the structures and free energies of protein-assisted membrane fusion. (C) 2014 The Authors. Published by Elsevier B.V. C1 [Rogers, David M.; Kent, Michael S.; Rempe, Susan B.] Sandia Natl Labs, Ctr Biol & Mat Sci, Albuquerque, NM 87185 USA. RP Rempe, SB (reprint author), Sandia Natl Labs, Ctr Biol & Mat Sci, POB 5800, Albuquerque, NM 87185 USA. EM slrempe@sandia.gov FU Sandia's LDRD program; DTRA; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors thank Aihua Zheng, Margaret Kielian, and Juan Vanegas for helpful discussions. This work was supported by Sandia's LDRD program and by DTRA. Sandia National Laboratories is a multiprogram laboratory operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 101 TC 4 Z9 4 U1 0 U2 19 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0005-2736 EI 0006-3002 J9 BBA-BIOMEMBRANES JI Biochim. Biophys. Acta-Biomembr. PD APR PY 2015 VL 1848 IS 4 BP 1041 EP 1052 DI 10.1016/j.bbamem.2014.12.018 PG 12 WC Biochemistry & Molecular Biology; Biophysics SC Biochemistry & Molecular Biology; Biophysics GA CC6ZZ UT WOS:000350518800017 PM 25559317 ER PT J AU Perez, D Uberuaga, BP Voter, AF AF Perez, Danny Uberuaga, Blas P. Voter, Arthur F. TI The parallel replica dynamics method - Coming of age SO COMPUTATIONAL MATERIALS SCIENCE LA English DT Article DE Computer simulations; Molecular dynamics; Accelerated molecular dynamics; Parallel replica dynamics ID TEMPERATURE-ACCELERATED DYNAMICS; SURFACE SELF-DIFFUSION; KINETIC MONTE-CARLO; MOLECULAR-DYNAMICS; INFREQUENT EVENTS; CHEMICAL-REACTIONS; RADIATION-DAMAGE; SIMULATIONS; SYSTEMS; APPROXIMATION AB Molecular dynamics (MD) - the numerical integration of atomistic equations of motion - is a workhorse of computational materials science. Indeed, MD can in principle be used to obtain any thermodynamic or kinetic quantity, without introducing approximation or assumptions beyond the adequacy of the interaction potential. It is therefore an extremely powerful and flexible tool to study materials with atomistic spatio-temporal resolution. These enviable qualities however come at a steep computational price, limiting the system sizes and simulation times that can be achieved in practice. While the size limitation can be efficiently addressed with massively parallel implementations of MD based on spatial decomposition strategies, allowing for the simulation of trillions of atoms, the same approach usually cannot extend the timescales much beyond microseconds. In this article, we discuss an alternative, parallel-in-time, strategy - the Parallel Replica Dynamics (ParRep) method - that aims at addressing the timescale limitation of MD for systems that evolve through rare state-to-state transitions. We review the formal underpinnings of the method, including recent developments showing it can provide arbitrarily accurate results for any definition of the states. When an adequate definition of the states is available, ParRep can simulate trajectories with a parallel speedup approaching the number of replicas used. We demonstrate the usefulness of ParRep by presenting different examples of materials simulations where access to long timescales was essential to study the physical regime of interest and discuss practical considerations that must be addressed to carry out these simulations. Sixteen years after its introduction, with a new understanding of its generality and ever increasing availability of parallel processing, the ParRep method is coming of age. (C) 2015 Elsevier B.V. All rights reserved. C1 [Perez, Danny; Voter, Arthur F.] Los Alamos Natl Lab, Theoret Div T 1, Los Alamos, NM 87545 USA. [Uberuaga, Blas P.] Los Alamos Natl Lab, Mat Sci & Technol Div MST 8, Los Alamos, NM 87545 USA. RP Perez, D (reprint author), Los Alamos Natl Lab, Theoret Div T 1, POB 1663, Los Alamos, NM 87545 USA. EM danny_perez@lanl.gov FU United States Department of Energy (U.S. DOE), Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division; Los Alamos National Laboratory (LANL) LDRD program; U.S. DOE [DE-AC52-O6NA25396] FX We are grateful to our collaborators Yalin Dong, Timothy Germann, Tony Lelievre, Claude Le Bris, Albert Lu, Sheng-Niang Luo, Mitchell Luskin, Enrique Martinez, Ashlie Martini, Chun-Wei Pao, Steven Stuart, and Sriram Swaminarayan. This work was supported by the United States Department of Energy (U.S. DOE), Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division and also reviews work supported by the Los Alamos National Laboratory (LANL) LDRD program. LANL is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. DOE, under contract DE-AC52-O6NA25396. NR 72 TC 13 Z9 14 U1 3 U2 32 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0927-0256 EI 1879-0801 J9 COMP MATER SCI JI Comput. Mater. Sci. PD APR 1 PY 2015 VL 100 SI SI BP 90 EP 103 DI 10.1016/j.commatsci.2014.12.011 PN B PG 14 WC Materials Science, Multidisciplinary SC Materials Science GA CC4ZQ UT WOS:000350366000002 ER PT J AU Mousseau, N Beland, LK Brommer, P El-Mellouhi, F Joly, JF Tsouaglo, GKN Restrepo, O Trochet, M AF Mousseau, Normand Beland, Laurent Karim Brommer, Peter El-Mellouhi, Fedwa Joly, Jean-Francois Tsouaglo, Gawonou Kokou N' Restrepo, Oscar Trochet, Mickael TI Following atomistic kinetics on experimental timescales with the kinetic Activation-Relaxation Technique SO COMPUTATIONAL MATERIALS SCIENCE LA English DT Article DE Defects; Diffusion; Activated dynamics; Kinetic Monte Carlo; Self assembly ID FINDING SADDLE-POINTS; IMPLANTED AMORPHOUS-SILICON; MONTE-CARLO; DIFFUSION MECHANISMS; MOLECULAR-DYNAMICS; SIMULATION; VACANCIES; CLUSTERS; SURFACE; STABILITY AB The properties of materials, even at the atomic level, evolve on macroscopic time scales. Following this evolution through simulation has been a challenge for many years. For lattice-based activated diffusion, kinetic Monte Carlo has turned out to be an almost perfect solution. Various accelerated molecular dynamical schemes, for their part, have allowed the study on long time scale of relatively simple systems. There is still a need, however, for methods able to handle complex materials such as alloys and disordered systems. Here, we review the kinetic Activation-Relaxation Technique (k-ART), one of a handful of off-lattice kinetic Monte Carlo methods, with on-the-fly cataloging, that have been proposed in the last few years. (C) 2014 Elsevier B.V. All rights reserved. C1 [Mousseau, Normand; Tsouaglo, Gawonou Kokou N'; Restrepo, Oscar; Trochet, Mickael] Univ Montreal, Dept Phys, Montreal, PQ H3C 3J7, Canada. [Mousseau, Normand] Univ Utrecht, Theoret Phys, Utrecht, Netherlands. [Brommer, Peter] Univ Warwick, Ctr Predict Modelling, Sch Engn, Coventry CV4 7AL, W Midlands, England. [Joly, Jean-Francois] Carleton Univ, Ottawa, ON K1S 5B6, Canada. [Beland, Laurent Karim] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN USA. [El-Mellouhi, Fedwa] Qatar Environm & Energy Res Inst, Doha, Qatar. [El-Mellouhi, Fedwa; Restrepo, Oscar] Texas A&M Univ Qatar, Doha, Qatar. RP Mousseau, N (reprint author), Univ Montreal, Dept Phys, CP 6128, Montreal, PQ H3C 3J7, Canada. EM normand.mousseau@umontreal.ca RI Brommer, Peter/B-5533-2008; Mousseau, Normand/E-3682-2013 OI Brommer, Peter/0000-0001-7312-9954; Mousseau, Normand/0000-0003-0575-7590 FU Canada Research Chairs program; Natural Sciences and Engineering Research Council of Canada (NSERC); Qatar National Research Fund (QNRF) through the National Priorities Research Program [NPRP 6-863-2-355]; Center for Defect Physics; Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences FX This work has been supported by the Canada Research Chairs program and by grants from the Natural Sciences and Engineering Research Council of Canada (NSERC). The work of OR and FE is supported by the Qatar National Research Fund (QNRF) through the National Priorities Research Program (NPRP 6-863-2-355). We are grateful to Calcul Quebec/Compute Canada (CQ/CC) for generous allocations of computer resources. NM would also like to thank Gerard Barkema and the Institute for Theoretical Physics of Utrecht University, where a good part of the article was written, for their hospitality. Some of LKB's work was supported by the Center for Defect Physics, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. NR 79 TC 7 Z9 7 U1 2 U2 25 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0927-0256 EI 1879-0801 J9 COMP MATER SCI JI Comput. Mater. Sci. PD APR 1 PY 2015 VL 100 SI SI BP 111 EP 123 DI 10.1016/j.commatsci.2014.11.047 PN B PG 13 WC Materials Science, Multidisciplinary SC Materials Science GA CC4ZQ UT WOS:000350366000004 ER PT J AU Beland, LK Osetsky, YN Stoller, RE Xu, HX AF Beland, Laurent Karim Osetsky, Yuri N. Stoller, Roger E. Xu, Haixuan TI Kinetic Activation-Relaxation Technique and Self-Evolving Atomistic Kinetic Monte Carlo: Comparison of on-the-fly Kinetic Monte Carlo algorithms SO COMPUTATIONAL MATERIALS SCIENCE LA English DT Article DE Off-lattice Kinetic Monte Carlo; Iron; Saddle-search; Vacancy aggregation; Interstitial-loop ID FINDING SADDLE-POINTS; TIME-SCALE; SIMULATION; DYNAMICS; SURFACES; DIFFUSION; CLUSTERS; IRON AB We present a comparison of the Kinetic Activation-Relaxation Technique (k-ART) and the Self-Evolving Atomistic Kinetic Monte Carlo (SEAKMC), two off-lattice, on-the-fly Kinetic Monte Carlo (KMC) techniques that were recently used to solve several materials science problems. We show that if the initial displacements are localized the dimer method and the Activation-Relaxation Technique nouveau provide similar performance. We also show that k-ART and SEAKMC, although based on different approximations, are in agreement with each other, as demonstrated by the examples of 50 vacancies in a 1950-atom Fe box and of interstitial loops in 16,000-atom boxes. Generally speaking, k-ART's treatment of geometry and flickers is more flexible, e.g. it can handle amorphous systems, and rigorous than SEAKMC's, while the later's concept of active volumes permits a significant speedup of simulations for the systems under consideration and therefore allows investigations of processes requiring large systems that are not accessible if not localizing calculations. (C) 2015 Elsevier B.V. All rights reserved. C1 [Beland, Laurent Karim; Osetsky, Yuri N.; Stoller, Roger E.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Xu, Haixuan] Univ Tennessee, Dept Mat Sci, Knoxville, TN 37996 USA. RP Xu, HX (reprint author), Univ Tennessee, Dept Mat Sci, Knoxville, TN 37996 USA. EM xhx@utk.edu RI Xu, Haixuan/C-9841-2009; OI Osetskiy, Yury/0000-0002-8109-0030 FU U.S. Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, "Center for Defect Physics,'' an Energy Frontier Research Center; Fonds Quebecois de recherche Nature et Technologies FX Research at the Oak Ridge National Laboratory sponsored by the U.S. Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, "Center for Defect Physics,'' an Energy Frontier Research Center. LKB acknowledges a fellowship awarded by the Fonds Quebecois de recherche Nature et Technologies. NR 66 TC 4 Z9 4 U1 3 U2 22 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0927-0256 EI 1879-0801 J9 COMP MATER SCI JI Comput. Mater. Sci. PD APR 1 PY 2015 VL 100 SI SI BP 124 EP 134 DI 10.1016/j.commatsci.2014.12.001 PN B PG 11 WC Materials Science, Multidisciplinary SC Materials Science GA CC4ZQ UT WOS:000350366000005 ER PT J AU Xu, HX Stoller, RE Beland, LK Osetsky, YN AF Xu, Haixuan Stoller, Roger E. Beland, Laurent K. Osetsky, Yuri N. TI Self-Evolving Atomistic Kinetic Monte Carlo simulations of defects in materials SO COMPUTATIONAL MATERIALS SCIENCE LA English DT Article DE Kinetic Monte Carlo; Self-Evolving Atomistic Kinetic Monte Carlo (SEAKMC); On-the-fly; Time scale; Active volume ID NEUTRON-IRRADIATION DAMAGE; ALPHA-IRON; DISLOCATION LOOPS; INFREQUENT EVENTS; INTERATOMIC POTENTIALS; HELIUM CLUSTERS; SADDLE-POINTS; TIME-SCALE; BCC IRON; DYNAMICS AB The recent development of on-the-fly atomistic kinetic Monte Carlo methods has led to an increased amount attention on the methods and their corresponding capabilities and applications. In this review, the framework and current status of Self-Evolving Atomistic Kinetic Monte Carlo (SEAKMC) are discussed. SEAKMC particularly focuses on defect interaction and evolution with atomistic details without assuming potential defect migration/interaction mechanisms and energies. The strength and limitation of using an active volume, the key concept introduced in SEAKMC, are discussed. Potential criteria for characterizing an active volume are discussed and the influence of active volume size on saddle point energies is illustrated. A procedure starting with a small active volume followed by larger active volumes was found to possess higher efficiency. Applications of SEAKMC, ranging from point defect diffusion, to complex interstitial cluster evolution, to helium interaction with tungsten surfaces, are summarized. A comparison of SEAKMC with molecular dynamics and conventional object kinetic Monte Carlo is demonstrated. Overall, SEAKMC is found to be complimentary to conventional molecular dynamics, especially when the harmonic approximation of transition state theory is accurate. However it is capable of reaching longer time scales than molecular dynamics and it can be used to systematically increase the accuracy of other methods such as object kinetic Monte Carlo. The challenges and potential development directions are also outlined. (C) 2014 Elsevier B.V. All rights reserved. C1 [Xu, Haixuan] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Stoller, Roger E.; Beland, Laurent K.; Osetsky, Yuri N.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN USA. RP Xu, HX (reprint author), Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. EM xhx@utk.edu RI Xu, Haixuan/C-9841-2009; OI Osetskiy, Yury/0000-0002-8109-0030 FU Center for Defect Physics, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [ERKCS99] FX Research at the Oak Ridge National Laboratory supported as part of the Center for Defect Physics, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number ERKCS99. NR 59 TC 3 Z9 3 U1 5 U2 25 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0927-0256 EI 1879-0801 J9 COMP MATER SCI JI Comput. Mater. Sci. PD APR 1 PY 2015 VL 100 SI SI BP 135 EP 143 DI 10.1016/j.commatsci.2014.12.026 PN B PG 9 WC Materials Science, Multidisciplinary SC Materials Science GA CC4ZQ UT WOS:000350366000006 ER PT J AU Nguyen, TD Plimpton, SJ AF Trung Dac Nguyen Plimpton, Steven J. TI Accelerating dissipative particle dynamics simulations for soft matter systems SO COMPUTATIONAL MATERIALS SCIENCE LA English DT Article DE Dissipative particle dynamics; LAMMPS; GPU acceleration; Hybrid CPU/GPU; Hybrid MPI/GPU; High-performance computing ID IMPLEMENTING MOLECULAR-DYNAMICS; MESOSCOPIC SIMULATION; INFREQUENT EVENTS; NUMBER GENERATORS; SOLVENT QUALITY; POISEUILLE FLOW; PERFORMANCE; RELAXATION; POTENTIALS; ALGORITHMS AB Dissipative particle dynamics (DPD) is a coarse-grained particle-based simulation method that offers microscopic-scale insights into soft matter systems. We present an efficient implementation of a DPD model for graphical processing units (GPUs). As implemented in the LAMMPS molecular dynamics package, it can run effectively on current-generation supercomputers which often have hybrid nodes containing multi-core CPUs and (one or more) GPUs. Using efficient communication of information between the CPUs and GPUs, DPD interactions can be computed on the GPU while other portions of a full simulation model (boundary conditions, constraints, bonded interactions, diagnostic calculations, etc.) can be performed on the CPU. Our GPU-enhanced runs show a speedup of up to 9.5x versus many-core CPU simulations, and can run scalably across thousands of compute nodes. We briefly discuss how the new GPU implementation was validated against the CPU version for thermodynamics, diffusion, and hydrodynamic behavior. We also highlight large-scale models which the faster DPD implementation has enabled, for studies of monolayer self-assembly and thin-film instabilities. (C) 2014 Elsevier B.V. All rights reserved. C1 [Trung Dac Nguyen] Oak Ridge Natl Lab, Natl Ctr Computat Sci, Oak Ridge, TN 37831 USA. [Plimpton, Steven J.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Nguyen, TD (reprint author), Oak Ridge Natl Lab, Natl Ctr Computat Sci, Oak Ridge, TN 37831 USA. EM ndactrung@gmail.com RI Nguyen, Trung/H-7008-2012 OI Nguyen, Trung/0000-0002-5076-264X FU Office of Advanced Scientific Computing Research, Office of Science, U.S. Department of Energy [DE-AC05-00OR22725]; UT-Battelle, LLC FX The GPU and CPU DPD models described here are part of the open-source LAMMPS distribution, available for download at http://lammps.sandia.gov. T.D.N. thanks W. M. Brown for helpful discussion regarding the implementation of the GPU package and Arnold N. Tharrington for comments on the random number generators on the GPU. This research used resources of the Leadership Computing Facility at Oak Ridge National Laboratory and was conducted under the auspices of the Office of Advanced Scientific Computing Research, Office of Science, U.S. Department of Energy under Contract No. DE-AC05-00OR22725 with UT-Battelle, LLC. NR 42 TC 3 Z9 3 U1 2 U2 28 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0927-0256 EI 1879-0801 J9 COMP MATER SCI JI Comput. Mater. Sci. PD APR 1 PY 2015 VL 100 SI SI BP 173 EP 180 DI 10.1016/j.commatsci.2014.10.068 PN B PG 8 WC Materials Science, Multidisciplinary SC Materials Science GA CC4ZQ UT WOS:000350366000010 ER PT J AU Lyakh, DI AF Lyakh, Dmitry I. TI An efficient tensor transpose algorithm for multicore CPU, Intel Xeon Phi, and NVidia Tesla GPU SO COMPUTER PHYSICS COMMUNICATIONS LA English DT Article DE Tensor transpose; Array reordering; Tensor contraction; Many-body theory; Electronic structure; Multireference; NVidia GPU; Intel Xeon Phi ID COUPLED-CLUSTER THEORY; CONTRACTION ENGINE; CHEMISTRY; IMPLEMENTATION; PERFORMANCE; FORMALISM; NWCHEM AB An efficient parallel tensor transpose algorithm is suggested for shared-memory computing units, namely, multicore CPU, Intel Xeon Phi, and NVidia GPU. The algorithm operates on dense tensors (multidimensional arrays) and is based on the optimization of cache utilization on x86 CPU and the use of shared memory on NVidia GPU. From the applied side, the ultimate goal is to minimize the overhead encountered in the transformation of tensor contractions into matrix multiplications in computer implementations of advanced methods of quantum many-body theory (e.g., in electronic structure theory and nuclear physics). A particular accent is made on higher-dimensional tensors that typically appear in the so-called multireference correlated methods of electronic structure theory. Depending on tensor dimensionality, the presented optimized algorithms can achieve an order of magnitude speedup on x86 CPUs and 2-3 times speedup on NVidia Tesla K2OX GPU with respect to the naive scattering algorithm (no memory access optimization). The tensor transpose routines developed in this work have been incorporated into a general-purpose tensor algebra library (TAL-SH). (C) 2014 Elsevier B.V. All rights reserved. C1 Oak Ridge Natl Lab, Natl Ctr Computat Sci, Oak Ridge, TN 37831 USA. RP Lyakh, DI (reprint author), Oak Ridge Natl Lab, Natl Ctr Computat Sci, Oak Ridge, TN 37831 USA. EM quant4me@gmail.com OI Lyakh, Dmitry/0000-0002-1851-2974 FU Air Force Office for Scientific Research; Office of Science of the US Department of Energy [DE-AC05-00OR22725]; National Science Foundation [1137097]; University of Tennessee FX The initial part of this work (open-source multi-CPU OpenMP implementation) was started during author's postdoctoral work at the Quantum Theory Project at the University of Florida (group of Prof. R.J. Bartlett) with the financial support from the Air Force Office for Scientific Research. The author is thankful for that opportunity. The computational resources of the HPC Center of the University of Florida are also appreciated. The rest of the work was accomplished in the Scientific Computing group (led by Dr. T. Straatsma) at the National Center for Computational Sciences at the Oak Ridge National Laboratory. This research used resources of the Oak Ridge Leadership Computing Facility at the Oak Ridge National Laboratory, which is supported by the Office of Science of the US Department of Energy under Contract No. DE-AC05-00OR22725. A part of the presented results was obtained using the computational resources of the Beacon project, supported by the National Science Foundation under Grant No. 1137097 and by the University of Tennessee: any opinions, findings, conclusions, or recommendations expressed in this material are those of the author and do not necessarily reflect the views of the National Science Foundation or the University of Tennessee. NR 29 TC 9 Z9 9 U1 1 U2 18 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0010-4655 EI 1879-2944 J9 COMPUT PHYS COMMUN JI Comput. Phys. Commun. PD APR PY 2015 VL 189 BP 84 EP 91 DI 10.1016/j.cpc.2014.12.013 PG 8 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA CC1FT UT WOS:000350087300010 ER PT J AU Xu, ZJ Li, DS Xu, W Devaraj, A Colby, R Thevuthasan, S Geiser, BP Larson, DJ AF Xu, Zhijie Li, Dongsheng Xu, Wei Devaraj, Arun Colby, Robert Thevuthasan, Suntharampillai Geiser, B. P. Larson, D. J. TI Simulation of heterogeneous atom probe tip shapes evolution during field evaporation using a level set method and different evaporation models SO COMPUTER PHYSICS COMMUNICATIONS LA English DT Article DE Atom probe tomography; Field evaporation; Evaporation model; Tip shape evolution; Level set; Interface tracking ID TRANSMISSION ELECTRON-MICROSCOPY; SPECIMEN PREPARATION; TOMOGRAPHY DATA; RECONSTRUCTION; PRECIPITATION; INTERFACES; THIN AB In atom probe tomography (APT), accurate reconstruction of the spatial positions of field evaporated ions from measured detector patterns depends upon a correct understanding of the dynamic tip shape evolution and evaporation laws of component atoms. Artifacts in APT reconstructions of heterogeneous materials can be attributed to the assumption of homogeneous evaporation of all the elements in the material in addition to the assumption of a steady state hemispherical dynamic tip shape evolution. A level set method-based specimen shape evolution model is developed in this study to simulate the evaporation of synthetic layered-structured APT tips. The simulation results of the shape evolution by the level set model qualitatively agree with the finite element method and the literature data using the finite difference method. The asymmetric evolving shape predicted by the level set model demonstrates the complex evaporation behavior of heterogeneous tip and the interface curvature can potentially lead to the artifacts in the APT reconstruction of such materials. Compared with other APT simulation methods, the new method provides smoother interface representation with the aid of the intrinsic sub-grid accuracy. Two evaporation models (linear and exponential evaporation laws) are implemented in the level set simulations and the effect of evaporation laws on the tip shape evolution is also presented. (C) 2015 Elsevier B.V. All rights reserved. C1 [Xu, Zhijie; Li, Dongsheng; Xu, Wei; Devaraj, Arun; Colby, Robert; Thevuthasan, Suntharampillai] Pacific NW Natl Lab, Richland, WA 99352 USA. [Geiser, B. P.; Larson, D. J.] CAMECA Instruments Inc, Madison, WI 53711 USA. RP Xu, ZJ (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM zhijie.xu@pnnl.gov; arun.devaraj@pnnl.gov RI Xu, Zhijie/A-1627-2009 OI Xu, Zhijie/0000-0003-0459-4531 FU DOE's Office of Biological and Environmental Research located at PNNL; William R. Wiley postdoctoral fellowship; LDRD; U.S. Department of Energy by Battelle [DE-AC06-76RL01830] FX The authors acknowledge the funding support from the LDRD-funded Chemical Imaging Initiative at Pacific Northwest National Laboratory, operated for the U.S. Department of Energy by Battelle under contract DE-AC06-76RL01830. A portion of the work was conducted in the William R. Wiley Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by DOE's Office of Biological and Environmental Research located at PNNL, and with the assistance of the William R. Wiley postdoctoral fellowship. NR 57 TC 4 Z9 4 U1 1 U2 12 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0010-4655 EI 1879-2944 J9 COMPUT PHYS COMMUN JI Comput. Phys. Commun. PD APR PY 2015 VL 189 BP 106 EP 113 DI 10.1016/j.cpc.2014.12.016 PG 8 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA CC1FT UT WOS:000350087300013 ER PT J AU Paul, S Aggarwal, C Thakur, JK Bandeppa, GS Khan, MA Pearson, LM Babnigg, G Giometti, CS Joachimiak, A AF Paul, Sangeeta Aggarwal, Chetana Thakur, Jyoti Kumar Bandeppa, G. S. Khan, Md. Aslam Pearson, Lauren M. Babnigg, Gyorgy Giometti, Carol S. Joachimiak, Andrzej TI Induction of Osmoadaptive Mechanisms and Modulation of Cellular Physiology Help Bacillus licheniformis Strain SSA 61 Adapt to Salt Stress SO CURRENT MICROBIOLOGY LA English DT Article ID POLYNUCLEOTIDE PHOSPHORYLASE; GLUTATHIONE-REDUCTASE; SUPEROXIDE-DISMUTASE; HYDROGEN-PEROXIDE; ESCHERICHIA-COLI; ACID; DEGRADATION; ADAPTATIONS; PROTEINS; CATALASE AB Bacillus licheniformis strain SSA 61, originally isolated from Sambhar salt lake, was observed to grow even in the presence of 25 % salt stress. Osmoadaptive mechanisms of this halotolerant B. licheniformis strain SSA 61, for long-term survival and growth under salt stress, were determined. Proline was the preferentially accumulated compatible osmolyte. There was also increased accumulation of antioxidants ascorbic acid and glutathione. Among the different antioxidative enzymes assayed, superoxide dismutase played the most crucial role in defense against salt-induced stress in the organism. Adaptation to stress by the organism involved modulation of cellular physiology at various levels. There was enhanced expression of known proteins playing essential roles in stress adaptation, such as chaperones DnaK and GroEL, and general stress protein YfkM and polynucleotide phosphorylase/polyadenylase. Proteins involved in amino acid biosynthetic pathway, ribosome structure, and peptide elongation were also overexpressed. Salt stress-induced modulation of expression of enzymes involved in carbon metabolism was observed. There was up-regulation of a number of enzymes involved in generation of NADH and NADPH, indicating increased cellular demand for both energy and reducing power. C1 [Paul, Sangeeta; Aggarwal, Chetana; Bandeppa, G. S.] Indian Agr Res Inst, Div Microbiol, New Delhi 10012, India. [Thakur, Jyoti Kumar] Indian Inst Soil Sci, Div Soil Biol, Bhopal 462038, Madhya Pradesh, India. [Khan, Md. Aslam] Jazan Univ, Fac Sci, Dept Biol, Jazan, Saudi Arabia. [Pearson, Lauren M.; Babnigg, Gyorgy; Giometti, Carol S.; Joachimiak, Andrzej] Argonne Natl Lab, Biosci Div, Argonne, IL 60439 USA. RP Paul, S (reprint author), Indian Agr Res Inst, Div Microbiol, New Delhi 10012, India. EM sangeeta_paul2003@yahoo.co.in FU NIGMS NIH HHS [U54 GM094585] NR 33 TC 0 Z9 0 U1 2 U2 6 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0343-8651 EI 1432-0991 J9 CURR MICROBIOL JI Curr. Microbiol. PD APR PY 2015 VL 70 IS 4 BP 610 EP 617 DI 10.1007/s00284-014-0761-y PG 8 WC Microbiology SC Microbiology GA CC3IR UT WOS:000350241000020 PM 25561404 ER PT J AU Nagase, T Rack, PD Noh, JH Egami, T AF Nagase, Takeshi Rack, Philip D. Noh, Joo Hyon Egami, Takeshi TI In-situ TEM observation of structural changes in nano-crystalline CoCrCuFeNi multicomponent high-entropy alloy (HEA) under fast electron irradiation by high voltage electron microscopy (HVEM) SO INTERMETALLICS LA English DT Article DE High-entropy alloys; Irradiation effects; In situ; Microstructure ID ORDER-DISORDER TRANSFORMATION; NI PHASE-DIAGRAM; HF-NB ALLOY; CO-CU-FE; METALLIC GLASSES; STABILITY; SYSTEM; AMORPHIZATION; TRANSITION; CHROMIUM AB The structural changes induced in a CoCrCuFeNi multicomponent nano-crystalline high-entropy alloy (HEA) under fast electron irradiation were investigated by in-situ transmission electron microscopy (TEM) using a high voltage electron microscope (HVEM). A fine-grained face centered cubic (fcc) single phase was obtained in the sputtered specimens. The fcc solid solution showed high phase stability against irradiation over a wide temperature range from 298 to 773 K, and remained as the main constituent phase even when the samples were irradiated up to 40 displacement per atom (dpa). Moreover, the irradiation did not seem to induce grain coarsening. This is the first report on the irradiation damage in 5-component HEA under MeV electron irradiation. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Nagase, Takeshi] Osaka Univ, Res Ctr Ultra High Voltage Electron Microscopy, Ibaraki, Osaka 5670047, Japan. [Nagase, Takeshi] Osaka Univ, Grad Sch Engn, Div Mat & Mfg Sci, Suita, Osaka 5650871, Japan. [Rack, Philip D.; Egami, Takeshi] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Rack, Philip D.; Noh, Joo Hyon; Egami, Takeshi] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Egami, Takeshi] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. RP Nagase, T (reprint author), Osaka Univ, Res Ctr Ultra High Voltage Electron Microscopy, 7-1 Mihogaoka, Ibaraki, Osaka 5670047, Japan. EM t-nagase@uhvem.osaka-u.ac.jp RI Nagase, Takeshi/M-1189-2015; OI Nagase, Takeshi/0000-0003-4868-0773; Rack, Philip/0000-0002-9964-3254 FU Ministry of Education, Culture, Sports, Science, and Technology, Japan; Joint Institute for Advanced Materials at the University of Tennessee; Oak Ridge National Laboratory; Department of Energy [DE-AC07-05ID14517] FX This work was supported in part by the Grants for Excellent Graduate Schools from the Ministry of Education, Culture, Sports, Science, and Technology, Japan. PDR and JHN acknowledge support from the Joint Institute for Advanced Materials at the University of Tennessee and the Oak Ridge National Laboratory. TE acknowledges support from the Department of Energy through the NEUP program, DE-AC07-05ID14517. NR 54 TC 12 Z9 12 U1 22 U2 116 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0966-9795 EI 1879-0216 J9 INTERMETALLICS JI Intermetallics PD APR PY 2015 VL 59 BP 32 EP 42 DI 10.1016/j.intermet.2014.12.007 PG 11 WC Chemistry, Physical; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Chemistry; Materials Science; Metallurgy & Metallurgical Engineering GA CC2OZ UT WOS:000350185800005 ER PT J AU Sargsyan, K Najm, HN Ghanem, R AF Sargsyan, K. Najm, H. N. Ghanem, R. TI On the Statistical Calibration of Physical Models SO INTERNATIONAL JOURNAL OF CHEMICAL KINETICS LA English DT Article ID SKELETAL MECHANISM GENERATION; UNCERTAINTY QUANTIFICATION; ARRHENIUS PARAMETERS; SHOCK-TUBE; CHEMICAL-SYSTEMS; BAYESIAN-ANALYSIS; RATE-COEFFICIENT; KINETIC-MODEL; N-HEPTANE; COMBUSTION AB We introduce a novel statistical calibration framework for physical models, relying on probabilistic embedding of model discrepancy error within the model. For clarity of illustration, we take the measurement errors out of consideration, calibrating a chemical model of interest with respect to a more detailed model, considered as truth for the present purpose. We employ Bayesian statistical methods for such model-to-model calibration and demonstrate their capabilities on simple synthetic models, leading to a well-defined parameter estimation problem that employs approximate Bayesian computation. The method is then demonstrated on two case studies for calibration of kinetic rate parameters for methane air chemistry, where ignition time information from a detailed elementary-step kinetic model is used to estimate rate coefficients of a simple chemical mechanism. We show that the calibrated model predictions fit the data and that uncertainty in these predictions is consistent in a mean-square sense with the discrepancy from the detailed model data. (C) 2015 Wiley Periodicals, Inc. C1 [Sargsyan, K.; Najm, H. N.] Sandia Natl Labs, Livermore, CA 94550 USA. [Ghanem, R.] Univ So Calif, Los Angeles, CA 90089 USA. RP Sargsyan, K (reprint author), Sandia Natl Labs, Livermore, CA 94550 USA. EM ksargsy@sandia.gov RI Ghanem, Roger/B-8570-2008 OI Ghanem, Roger/0000-0002-1890-920X FU Scientific Discovery through Advanced Computing (SciDAC) program - U.S. Department of Energy, Office of Science, Advanced Scientific Computing Research; US Department of Energy (DOE), Office of Basic Energy Sciences (BES) Division of Chemical Sciences, Geosciences, and Biosciences; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94-AL85000] FX KS and RG acknowledge support for this work through the Scientific Discovery through Advanced Computing (SciDAC) program funded by the U.S. Department of Energy, Office of Science, Advanced Scientific Computing Research. HNN acknowledges support for this work through the US Department of Energy (DOE), Office of Basic Energy Sciences (BES) Division of Chemical Sciences, Geosciences, and Biosciences. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94-AL85000. NR 85 TC 5 Z9 5 U1 4 U2 14 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0538-8066 EI 1097-4601 J9 INT J CHEM KINET JI Int. J. Chem. Kinet. PD APR PY 2015 VL 47 IS 4 BP 246 EP 276 DI 10.1002/kin.20906 PG 31 WC Chemistry, Physical SC Chemistry GA CC4DO UT WOS:000350301200003 ER PT J AU Paul, TC Morshed, AKMM Fox, EB Khan, JA AF Paul, Titan C. Morshed, A. K. M. M. Fox, Elise B. Khan, Jamil A. TI Experimental investigation of natural convection heat transfer of Al2O3 Nanoparticle Enhanced Ionic Liquids (NEILs) SO INTERNATIONAL JOURNAL OF HEAT AND MASS TRANSFER LA English DT Article DE Nanoparticle Enhanced Ionic Liquid (NEILs); Density; Viscosity; Heat capacity; Thermal conductivity; Convective heat transfer coefficient; Nusselt number; Rayleigh number ID METALLIC NANOPARTICLES; THERMAL-STABILITY; TRANSFER FLUIDS; NANOFLUIDS; STABILIZATION; PERFORMANCE; SOLVATION; PARTICLES; CHEMISTRY; SOLVENTS AB Experimental investigations were carried out regarding natural convection heat transfer of Nanoparticle Enhanced Ionic Liquids (NEILs) in rectangular enclosures of two different sizes with dimensions length x width x height, 50 x 50 x 50 mm and 50 x 50 x 75 mm in heated from below. The NEILs were synthesized by dispersing different wt% (0.5, 1.0, and 2.5) of aluminum oxide (Al2O3) nanoparticles of two different particle shapes (spherical and whiskers) into N-butyl-N-methylpyrrolidinium bis{(trifluoromethyl)sulfonyl} imide, ([C(4)mpyrr][NTf2]) ionic liquid (IL). Heat transfer related thermophysical properties, i.e. density, viscosity, thermal conductivity, and heat capacity of base IL and NEILs were also measured and reported. The experimental measurement shows enhanced density, thermal conductivity, viscosity, and heat capacity of NEILs compared to the base IL and they increase with the nanoparticle concentration. However natural convection heat transfer coefficient was observed to deteriorate for the NEILs compared to the base IL irrespective of the shapes of the particles and aspect ratio of the enclosure and the deterioration increases with the increase of nanoparticle concentration. Interestingly spherical Al2O3 NEILs was observed to affect more adversely compared to the whiskers Al2O3 NEILs. The observed degradation of the heat transfer performance of the NEILs could not fully be explained by the change of thermophysical properties, which indicates that other factors may play significant roles in this phenomenon and the possible reasons of the degradation is discussed in this paper. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Paul, Titan C.; Morshed, A. K. M. M.; Khan, Jamil A.] Univ S Carolina, Dept Mech Engn, Columbia, SC 29208 USA. [Fox, Elise B.] Savannah River Natl Lab, Aiken, SC USA. RP Khan, JA (reprint author), Univ S Carolina, Dept Mech Engn, Columbia, SC 29208 USA. EM khan@cec.sc.edu FU Department of Energy (DOE) Solar Energy Technology Program; U.S. Department of Energy [DEAC09-08SR22470] FX The financial support for this research is from the Department of Energy (DOE) Solar Energy Technology Program. Savannah River National Laboratory is operated by Savannah River Nuclear Solutions. This document was prepared in conjunction with work accomplished under Contract No. DEAC09-08SR22470 with the U.S. Department of Energy. NR 36 TC 2 Z9 2 U1 1 U2 23 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0017-9310 EI 1879-2189 J9 INT J HEAT MASS TRAN JI Int. J. Heat Mass Transf. PD APR PY 2015 VL 83 BP 753 EP 761 DI 10.1016/j.ijheatmasstransfer.2014.12.067 PG 9 WC Thermodynamics; Engineering, Mechanical; Mechanics SC Thermodynamics; Engineering; Mechanics GA CC1CY UT WOS:000350080000073 ER PT J AU Pokharel, R Lind, J Li, SF Kenesei, P Lebensohn, RA Suter, RM Rollett, AD AF Pokharel, Reeju Lind, Jonathan Li, Shiu Fai Kenesei, Peter Lebensohn, Ricardo A. Suter, Robert M. Rollett, Anthony D. TI In-situ observation of bulk 3D grain evolution during plastic deformation in polycrystalline Cu SO INTERNATIONAL JOURNAL OF PLASTICITY LA English DT Article DE Microstructures; Crystal plasticity; Polycrystalline material; Non-destructive evaluation; High-energy X-ray diffraction microscopy ID X-RAY-DIFFRACTION; ELECTRON BACKSCATTER DIFFRACTION; TEXTURE EVOLUTION; ELASTIC STRAINS; PART 1; ORIENTATION; MICROSCOPY; COPPER; RECRYSTALLIZATION; MICROSTRUCTURE AB We present a non-destructive in-situ measurement of three-dimensional (3D) microstructure evolution of 99.995% pure polycrystalline copper during tensile loading using synchrotron radiation. Spatially resolved three-dimensional crystallographic orientation fields are reconstructed from the measured diffraction data obtained from a near-field high-energy X-ray diffraction microscopy (nf-HEDM), and the evolution of about 5000 3D bulk grains is tracked through multiple stages of deformation. Spatially resolved observation of macroscopic texture change, anisotropic deformation development, and the correspondence of different crystallographic parameters to defect accumulation are illustrated. Moreover, correlations between different crystallographic parameters, such as crystal rotation evolution, short- and long-range orientation gradient development, microstructural features, and grain size effects are investigated. The current state of data mining tools available to analyze large and complicated diffraction data is presented and challenges associated with extracting meaningful information from these datasets are discussed. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Pokharel, Reeju; Lind, Jonathan; Suter, Robert M.; Rollett, Anthony D.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Lind, Jonathan; Li, Shiu Fai] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Pokharel, Reeju; Lebensohn, Ricardo A.] Los Alamos Natl Lab, Mat Sci & Technol Div, Los Alamos, NM 87544 USA. [Kenesei, Peter] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Pokharel, R (reprint author), Los Alamos Natl Lab, Mat Sci & Technol Div, POB 1663, Los Alamos, NM 87544 USA. EM reeju@lanl.gov RI Lebensohn, Ricardo/A-2494-2008; Suter, Robert/P-2541-2014; Rollett, Anthony/A-4096-2012 OI Lebensohn, Ricardo/0000-0002-3152-9105; Suter, Robert/0000-0002-0651-0437; Rollett, Anthony/0000-0003-4445-2191 FU US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DESC0002001]; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; Los Alamos National Laboratory's Directed Research and Development (LDRD-DR Project) [20140114DR]; Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; National Science Foundation [DMR080072]; National Energy Research Scientific Computing Center - Office of Science of the US Department of Energy [DE-AC02-05CH11231] FX This research was supported by the US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, under Award DESC0002001. Use of the Advanced Photon Source was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. Partial support from Los Alamos National Laboratory's Directed Research and Development (LDRD-DR Project 20140114DR) is also acknowledged. Part of this work was performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. This Research was also supported in part by the National Science Foundation through XSEDE resources provided by Texas Advanced Computing Center under Grant No. DMR080072, and in part by the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the US Department of Energy under Contract No. DE-AC02-05CH11231. NR 53 TC 12 Z9 12 U1 3 U2 31 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0749-6419 EI 1879-2154 J9 INT J PLASTICITY JI Int. J. Plast. PD APR PY 2015 VL 67 BP 217 EP 234 DI 10.1016/j.ijplas.2014.10.013 PG 18 WC Engineering, Mechanical; Materials Science, Multidisciplinary; Mechanics SC Engineering; Materials Science; Mechanics GA CC7GC UT WOS:000350534700011 ER PT J AU Rodriguez, JN Hwang, WJ Horn, J Landsman, TL Boyle, A Wierzbicki, MA Hasan, SM Follmer, D Bryant, J Small, W Maitland, DJ AF Rodriguez, Jennifer N. Hwang, Wonjun Horn, John Landsman, Todd L. Boyle, Anthony Wierzbicki, Mark A. Hasan, Sayyeda M. Follmer, Douglas Bryant, Jesse Small, Ward Maitland, Duncan J. TI Design and biocompatibility of endovascular aneurysm filling devices SO JOURNAL OF BIOMEDICAL MATERIALS RESEARCH PART A LA English DT Review DE intracranial aneurysm; shape memory polymer; aneurysm filling device; endovascular; embolization ID SINGLE-CENTER EXPERIENCE; GUGLIELMI DETACHABLE COILS; BARE PLATINUM COILS; CEREBRAL ARTERIOVENOUS-MALFORMATIONS; INTRACRANIAL SACCULAR ANEURYSMS; INITIAL CLINICAL-EXPERIENCE; HYDROGEL-COATED COILS; WALL SHEAR-STRESS; FOLLOW-UP; ARTERY ANEURYSMS AB The rupture of an intracranial aneurysm, which can result in severe mental disabilities or death, affects approximately 30,000 people in the United States annually. The traditional surgical method of treating these arterial malformations involves a full craniotomy procedure, wherein a clip is placed around the aneurysm neck. In recent decades, research and device development have focused on new endovascular treatment methods to occlude the aneurysm void space. These methods, some of which are currently in clinical use, utilize metal, polymeric, or hybrid devices delivered via catheter to the aneurysm site. In this review, we present several such devices, including those that have been approved for clinical use, and some that are currently in development. We present several design requirements for a successful aneurysm filling device and discuss the success or failure of current and past technologies. We also present novel polymeric-based aneurysm filling methods that are currently being tested in animal models that could result in superior healing. (c) 2014 Wiley Periodicals, Inc. J Biomed Mater Res Part A 103A: 1577-1594, 2015. C1 [Rodriguez, Jennifer N.; Hwang, Wonjun; Horn, John; Landsman, Todd L.; Boyle, Anthony; Wierzbicki, Mark A.; Hasan, Sayyeda M.; Follmer, Douglas; Bryant, Jesse; Maitland, Duncan J.] Texas A&M Univ, Dept Biomed Engn, College Stn, TX 77843 USA. [Small, Ward] Lawrence Livermore Natl Lab, Div Chem Sci, Livermore, CA USA. RP Maitland, DJ (reprint author), Texas A&M Univ, Dept Biomed Engn, 3120 TAMU, College Stn, TX 77843 USA. EM djmaitland@tamu.edu FU National Institutes of Health/National Institute of Biomedical Imaging and Bioengineering [R01EB000462]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX Contract grant sponsor: National Institutes of Health/National Institute of Biomedical Imaging and Bioengineering; contract grant number: R01EB000462; Contract grant sponsor: The auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory; contract grant number: DE-AC52-07NA27344 NR 151 TC 2 Z9 2 U1 1 U2 28 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1549-3296 EI 1552-4965 J9 J BIOMED MATER RES A JI J. Biomed. Mater. Res. Part A PD APR PY 2015 VL 103 IS 4 BP 1577 EP 1594 DI 10.1002/jbm.a.35271 PG 18 WC Engineering, Biomedical; Materials Science, Biomaterials SC Engineering; Materials Science GA CC5JQ UT WOS:000350395300027 PM 25044644 ER PT J AU Abreu-Sepulveda, MA Harun, NF Hackett, G Hagen, A Tucker, D AF Abreu-Sepulveda, Maria A. Harun, Nor Farida Hackett, Gregory Hagen, Anke Tucker, David TI Accelerated Degradation for Hardware in the Loop Simulation of Fuel Cell-Gas Turbine Hybrid System SO JOURNAL OF FUEL CELL SCIENCE AND TECHNOLOGY LA English DT Article ID CURRENT LOAD; CATHODE; SOFC; TEMPERATURE; PERFORMANCE; IMPEDANCE; BEHAVIOR AB The U.S. Department of Energy (DOE)-National Energy Technology Laboratory (NETL) in Morgantown, WV has developed the hybrid performance (HyPer) project in which a solid oxide fuel cell (SOFC) one-dimensional (1D), real-time operating model is coupled to a gas turbine hardware system by utilizing hardware-in-the-loop simulation. To assess the long-term stability of the SOFC part of the system, electrochemical degradation due to operating conditions such as current density and fuel utilization have been incorporated into the SOFC model and successfully recreated in real time. The mathematical expression for degradation rate was obtained through the analysis of empirical voltage versus time plots for different current densities and fuel utilizations. C1 [Abreu-Sepulveda, Maria A.; Hackett, Gregory; Tucker, David] US DOE, Natl Energy Technol Lab, Morgantown, WV 26507 USA. [Harun, Nor Farida] McMaster Univ, Dept Chem Engn, Hamilton, ON L8S 4L7, Canada. [Hagen, Anke] Tech Univ Denmark, Dept Energy Convers, DK-4000 Roskilde, Denmark. RP Abreu-Sepulveda, MA (reprint author), US DOE, Natl Energy Technol Lab, 3610 Collins Ferry Rd, Morgantown, WV 26507 USA. EM maria.abreu-sepulveda@contr.netl.doe.gov; adfarimie@yahoo.com; gregory.hackett@netl.doe.gov; anke@dtu.dk; david.tucker@netl.doe.gov OI Hagen, Anke/0000-0003-2001-8040 FU U.S. Department of Energy Cross-cutting Research program; U.S. DOE Mickey Leland Energy Fellowship Program FX This work was funded by the U.S. Department of Energy Cross-cutting Research program, administered through the National Energy Technology Laboratory and partially funded by the U.S. DOE Mickey Leland Energy Fellowship Program. NR 13 TC 0 Z9 0 U1 0 U2 12 PU ASME PI NEW YORK PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA SN 1550-624X EI 1551-6989 J9 J FUEL CELL SCI TECH JI J. Fuel Cell Sci. Technol. PD APR PY 2015 VL 12 IS 2 AR 021001 DI 10.1115/1.4028953 PG 7 GA CC6RR UT WOS:000350495700001 ER PT J AU Shcherbak, L Kopach, O Fochuk, P Bolotnikov, AE James, RB AF Shcherbak, L. Kopach, O. Fochuk, P. Bolotnikov, A. E. James, R. B. TI Empirical Correlations Between the Arrhenius' Parameters of Impurities' Diffusion Coefficients in CdTe Crystals SO JOURNAL OF PHASE EQUILIBRIA AND DIFFUSION LA English DT Article DE Arrhenius' equation; CdTe; compensation effect; impurities diffusion; Meyer-Neldel rule ID MEYER-NELDEL RULE; DOPED CADMIUM TELLURIDE; SELF-DIFFUSION; INTRINSIC DEFECTS; THIN-FILMS; COMPENSATION; SOLUBILITY; AG; CU; SEMICONDUCTORS AB Understanding of self- and dopant-diffusion in semiconductor devices is essential to our being able to assure the formation of well-defined doped regions. In this paper, we compare obtained in the literature up to date the Arrhenius' parameters (D=D (0)exp(-Delta E (a)/kT)) of point-defect diffusion coefficients and the I-VII groups impurities in CdTe crystals and films. We found that in the diffusion process there was a linear dependence between the pre-exponential factor, D (0), and the activation energy, Delta E (a), of different species: This was evident in the self-diffusivity and isovalent impurity Hg diffusivity as well as for the dominant IIIA and IVA groups impurities and Chlorine, except for the fast diffusing elements (e.g., Cu and Ag), chalcogens O, S, and Se, halogens I and Br as well as the transit impurities Mn, Co, Fe. Reasons of the lack of correspondence of the data to compensative dependence are discussed. C1 [Shcherbak, L.; Kopach, O.; Fochuk, P.] Chernivtsy Natl Univ, UA-58012 Chernovtsy, Ukraine. [Bolotnikov, A. E.; James, R. B.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Shcherbak, L (reprint author), Chernivtsy Natl Univ, 2 Kotsiubynskoho Str, UA-58012 Chernovtsy, Ukraine. EM l.shcherbak@chnu.edu.ua; o.kopach@chnu.edu.ua RI Fochuk, Petro/D-9409-2016; Kopach, Oleh/C-3993-2017; Shcherbak, Larysa/D-7332-2017 OI Fochuk, Petro/0000-0002-4149-4882; Kopach, Oleh/0000-0002-1513-5261; Shcherbak, Larysa/0000-0003-1048-9818 FU Science@Technology Center of Ukraine [P406]; U. S. Department of Energy; DOE/NNSA MNN RD FX This work is partly supported by the Science@Technology Center of Ukraine under the project P406 with U. S. Department of Energy, and by DOE/NNSA MNN R&D. The authors wish to thank Dr. D. Shaw, for his time spent in discussions and his useful advices. NR 73 TC 2 Z9 2 U1 1 U2 15 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1547-7037 EI 1863-7345 J9 J PHASE EQUILIB DIFF JI J. Phase Equilib. Diffus. PD APR PY 2015 VL 36 IS 2 BP 99 EP 109 DI 10.1007/s11669-015-0364-8 PG 11 WC Chemistry, Physical; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Chemistry; Materials Science; Metallurgy & Metallurgical Engineering GA CD1AV UT WOS:000350806900003 ER PT J AU Somerday, BP Barney, M AF Somerday, Brian P. Barney, Monica TI Measurement of Fatigue Crack Growth Relationships in Hydrogen Gas for Pressure Swing Adsorber Vessel Steels SO JOURNAL OF PRESSURE VESSEL TECHNOLOGY-TRANSACTIONS OF THE ASME LA English DT Article ID GASEOUS-HYDROGEN; PIPELINE STEEL AB Hydrogen-assisted fatigue crack growth rates (da/dN) were measured for SA516 Grade 70 steel as a function of stress-intensity factor range (Delta K) and load-cycle frequency to provide life-prediction data relevant to pressure swing adsorber (PSA) vessels. For Delta K values up to 18.5 MPa m(1/2), the baseline da/dN versus Delta K relationship measured at 1Hz in 2.8 MPa hydrogen gas represents an upper bound with respect to crack growth rates measured at lower frequency. However, at higher Delta K values, baseline da/dN data must be corrected to account for modestly higher crack growth rates at the lower frequencies relevant to PSA vessel operation. C1 [Somerday, Brian P.] Sandia Natl Labs, Livermore, CA 94550 USA. [Barney, Monica] Chevron Energy Technol Co, Richmond, CA 94801 USA. RP Somerday, BP (reprint author), Sandia Natl Labs, 7011 East Ave, Livermore, CA 94550 USA. EM bpsomer@sandia.gov; MBarney@chevron.com FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The assistance of Ken Lee in conducting the fatigue crack growth tests in hydrogen gas as well as Andy Gardea, Jeff Chames, and Ryan Nishimoto in performing metallography and microscopy is gratefully acknowledged. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. Initial project input and ongoing technical review from David Cooke and Ned Niccolls (Chevron) are greatly appreciated. NR 14 TC 0 Z9 0 U1 3 U2 9 PU ASME PI NEW YORK PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA SN 0094-9930 EI 1528-8978 J9 J PRESS VESS-T ASME JI J. Press. Vessel Technol.-Trans. ASME PD APR PY 2015 VL 137 IS 2 AR 021406 DI 10.1115/1.4028349 PG 7 WC Engineering, Mechanical SC Engineering GA CC6FM UT WOS:000350460400016 ER PT J AU Wang, YL Sham, TL Jetter, RI AF Wang, Yanli Sham, T. -L. Jetter, Robert I. TI Alloy 617 Creep-Fatigue Damage Evaluation Using Specimens With Strain Redistribution SO JOURNAL OF PRESSURE VESSEL TECHNOLOGY-TRANSACTIONS OF THE ASME LA English DT Article ID NICKEL-ALLOY AB The simplified model test (SMT) method is an alternate approach to determine the cyclic life at elevated temperature. It is based on the use of creep-fatigue hold time test data from test specimens with elastic follow-up conservatively designed to bound the response of general structural components. In this paper, the previously documented development of the SMT approach and applicable restrictions are reviewed; the design of the Alloy 617 SMT specimen, measurement issues and constraints are presented; initial test results and their application to a prototypic design curve are presented; and further testing and analysis for ASME code incorporation are discussed. C1 [Wang, Yanli; Sham, T. -L.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Jetter, Robert I.] RI Jetter Consulting, Pebble Beach, CA 93953 USA. RP Wang, YL (reprint author), Oak Ridge Natl Lab, 1 Bethel Valley Rd,POB 2008,MS 6083, Oak Ridge, TN 37831 USA. EM wangy3@ornl.gov; shamt@ornl.gov; bjetter@sbcglobal.net FU U.S. Department of Energy (DOE) [DE-AC05-00OR22725]; Oak Ridge National Laboratory FX The research was sponsored by the U.S. Department of Energy (DOE), under Contract No. DE-AC05-00OR22725 with Oak Ridge National Laboratory, managed and operated by UT-Battelle, LLC. Programmatic direction was provided by the DOE Office of Nuclear Energy, Office of Advanced Reactor Technologies. NR 9 TC 0 Z9 0 U1 3 U2 8 PU ASME PI NEW YORK PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA SN 0094-9930 EI 1528-8978 J9 J PRESS VESS-T ASME JI J. Press. Vessel Technol.-Trans. ASME PD APR PY 2015 VL 137 IS 2 AR 021402 DI 10.1115/1.4028054 PG 6 WC Engineering, Mechanical SC Engineering GA CC6FM UT WOS:000350460400012 ER PT J AU Addy, NJ Kiliccote, S Callaway, DS Mathieu, JL AF Addy, Nathan J. Kiliccote, Sila Callaway, Duncan S. Mathieu, Johanna L. TI How Baseline Model Implementation Choices Affect Demand Response Assessments SO JOURNAL OF SOLAR ENERGY ENGINEERING-TRANSACTIONS OF THE ASME LA English DT Article ID COMMERCIAL BUILDINGS; SAVINGS AB The performance of buildings participating in demand response (DR) programs is usually evaluated with baseline models, which predict what electric demand would have been if a DR event had not been called. Different baseline models produce different results. Moreover, modelers implementing the same baseline model often make different model implementation choices producing different results. Using real data from a DR program in CA and a regression-based baseline model, which relates building demand to time of week, outdoor air temperature, and building operational mode, we analyze the effect of model implementation choices on DR shed estimates. Results indicate strong sensitivities to the outdoor air temperature data source and bad data filtration methods, with standard deviations of differences in shed estimates of approximate to 20-30 kW, and weaker sensitivities to demand/temperature data resolution, data alignment, and methods for determining when buildings are occupied, with standard deviations of differences in shed estimates of approximate to 2-5 kW. C1 [Addy, Nathan J.; Kiliccote, Sila] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Callaway, Duncan S.] Univ Calif Berkeley, Energy & Resources Grp, Berkeley, CA 94720 USA. [Mathieu, Johanna L.] Univ Michigan, Dept Elect Engn & Comp Sci, Ann Arbor, MI 48109 USA. RP Mathieu, JL (reprint author), Univ Michigan, Dept Elect Engn & Comp Sci, 1301 Beal Ave, Ann Arbor, MI 48109 USA. EM nathan.addy@gmail.com; skiliccote@lbl.gov; dcal@berkeley.edu; jlmath@umich.edu FU Demand Response Research Center by California Energy Commission, Public Interest Energy Research (PIER) Program [500-03-026]; U.S. Department of Energy [DE-AC02-05CH11231]; Pacific Gas and Electric Company through Demand Response and Emerging Technologies Programs FX The authors would like to thank Pacific Gas and Electric Company for providing the electric demand data. This work was sponsored in part by the Demand Response Research Center, which is funded by the California Energy Commission, Public Interest Energy Research (PIER) Program, under Work for Others Contract No. 500-03-026 and by the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. This work was also partially funded by Pacific Gas and Electric Company through their Demand Response and Emerging Technologies Programs. NR 19 TC 3 Z9 3 U1 1 U2 7 PU ASME PI NEW YORK PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA SN 0199-6231 EI 1528-8986 J9 J SOL ENERG-T ASME JI J. Sol. Energy Eng. Trans.-ASME PD APR PY 2015 VL 137 IS 2 AR UNSP 021008 DI 10.1115/1.4028478 PG 6 WC Energy & Fuels; Engineering, Mechanical SC Energy & Fuels; Engineering GA CC7TP UT WOS:000350571600008 ER PT J AU Griffith, DT Moya, AC Ho, CK Hunter, PS AF Griffith, D. Todd Moya, Adam C. Ho, Clifford K. Hunter, Patrick S. TI Structural Dynamics Testing and Analysis for Design Evaluation and Monitoring of Heliostats SO JOURNAL OF SOLAR ENERGY ENGINEERING-TRANSACTIONS OF THE ASME LA English DT Article AB Heliostat vibrations due to wind loading can degrade optical pointing accuracy while fatiguing the structural components. This paper reports the use of structural dynamic measurements for design evaluation and monitoring of heliostat vibrations. A heliostat located at the national solar thermal testing facility (NSTTF) at Sandia National Laboratories in Albuquerque, New Mexico, has been instrumented to measure its modes of vibration, strain and displacements under wind loading. The information gained from these tests will be used to evaluate and improve structural models that predict the motions/deformations of the heliostat due to gravitational and dynamic wind loadings. These deformations can cause optical errors and motions that degrade the performance of the heliostat. The main contributions of this work include: (1) demonstration of the role of structural dynamic tests (also known as modal tests) to provide a characterization of the important dynamics of the heliostat structure as they relate to durability and optical accuracy, (2) the use of structural dynamic tests to provide data to evaluate and improve the accuracy of computer-based design models, and (3) the selection of sensors and data-processing techniques that are appropriate for long-term monitoring of heliostat motions. This work also demonstrates the first measurements of rigid body modes of vibration associated with heliostat drive (azimuth and elevation) mechanisms, which are important structural dynamic response characteristics in dynamic design of heliostats. C1 [Griffith, D. Todd; Hunter, Patrick S.] Sandia Natl Labs, Engn Sci Ctr, Albuquerque, NM 87185 USA. [Moya, Adam C.; Ho, Clifford K.] Concentrating Solar Technol Dept, Albuquerque, NM 87185 USA. RP Griffith, DT (reprint author), Sandia Natl Labs, Engn Sci Ctr, POB 5800, Albuquerque, NM 87185 USA. EM dgriffi@sandia.gov FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors would like to thank a number of people from Sandia Labs who made significant contributions to the planning and execution of these tests. Cheryl Ghanbari helped in the early test planning and logistics and helped identify a suitable heliostat for these tests. Ron Briggs performed much of the pretest safety analysis. Ernie Trujillo provided significant support of sensor installation and operation of the heliostat and portable lift. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 11 TC 0 Z9 0 U1 1 U2 7 PU ASME PI NEW YORK PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA SN 0199-6231 EI 1528-8986 J9 J SOL ENERG-T ASME JI J. Sol. Energy Eng. Trans.-ASME PD APR PY 2015 VL 137 IS 2 AR 021010 DI 10.1115/1.4028561 PG 10 WC Energy & Fuels; Engineering, Mechanical SC Energy & Fuels; Engineering GA CC7TP UT WOS:000350571600010 ER PT J AU Yuan, JK Christian, JM Ho, CK AF Yuan, James K. Christian, Joshua M. Ho, Clifford K. TI Compensation of Gravity Induced Heliostat Deflections for Improved Optical Performance SO JOURNAL OF SOLAR ENERGY ENGINEERING-TRANSACTIONS OF THE ASME LA English DT Article AB Heliostat optical performance can be affected by both wind and gravity induced deflections in the mirror support structure. These effects can result in decreased energy collection efficiency, depending on the magnitude of structural deflections, heliostat orientation and field position, and sun position. This paper presents a coupled modeling approach to evaluate the effects of gravity loading on heliostat optical performance, considering two heliostat designs: The National Solar Thermal Test Facility (NSTTF) heliostat and the Advanced Thermal Systems (ATS) heliostat. Deflections under gravitational loading were determined using finite element analysis (FEA) in ANSYS MECHANICAL, and the resulting deformed heliostat geometry was analyzed using Breault APEX optical engineering software to evaluate changes in beam size and shape. Optical results were validated against images of actual beams produced by each respective heliostat, measured using the Beam Characterization System (BCS) at Sandia National Laboratories. Simulated structural deflections in both heliostats were found to have visible impacts on beam shape, with small but quantifiable changes in beam power distribution. In this paper, the combined FEA and optical analysis method is described and validated, as well as a method for modeling heliostats subjected to gravitational deflection and canted in-field, for which mirror positions may not be known rigorously. Furthermore, a modified, generalized construction method is proposed and analyzed for the ATS heliostat, which was found to give consistent improvements in beam shape and up to a 4.1% increase in annual incident power weighted intercept (AIPWI). C1 [Yuan, James K.; Christian, Joshua M.; Ho, Clifford K.] Sandia Natl Labs, Concentrating Solar Technol Dept, Albuquerque, NM 87185 USA. RP Yuan, JK (reprint author), Sandia Natl Labs, Concentrating Solar Technol Dept, POB 5800, Albuquerque, NM 87185 USA. FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 6 TC 0 Z9 0 U1 2 U2 13 PU ASME PI NEW YORK PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA SN 0199-6231 EI 1528-8986 J9 J SOL ENERG-T ASME JI J. Sol. Energy Eng. Trans.-ASME PD APR PY 2015 VL 137 IS 2 AR 021016 DI 10.1115/1.4028938 PG 8 WC Energy & Fuels; Engineering, Mechanical SC Energy & Fuels; Engineering GA CC7TP UT WOS:000350571600016 ER PT J AU Foito, A Hackett, CA Byrne, SL Stewart, D Barth, S AF Foito, Alexandre Hackett, Christine Anne Byrne, Stephen L. Stewart, Derek Barth, Susanne TI Quantitative trait loci analysis to study the genetic regulation of non-polar metabolites in perennial ryegrass SO METABOLOMICS LA English DT Article DE Lolium perenne; Metabolomics; QTL ID CHAIN FATTY ALCOHOLS; DIET COMPOSITION MARKERS; LOLIUM-PERENNE; ACID-COMPOSITION; N-ALKANES; HUMAN HEALTH; IN-VITRO; FISH-OIL; METABOLOMICS; QUALITY AB In recent years advances in quantitative trait loci (QTL) mapping of complex metabolomics traits have been made in plants. This study is a two-phase experiment in which we have profiled transesterified non-polar metabolites in a Lolium perenne population consisting of parents, F1 and 325 F2 genotypes. These were grown in a replicated field trial, then analysed in batches by a targeted approach using gas-chromatography mass spectrometry (GC-MS), which identified 17 metabolites. The metabolite data was analysed using a mixed model that included random effects of field replicate, laboratory batch and technical replication to derive genotype means for QTL mapping. Using a linkage map of 326 markers, mainly Diversity Array Technology markers, QTLs were detected for seven of the metabolites. The most heritable metabolite was octacosanol, where a single QTL on linkage group four explained 42 % of the trait variance. C1 [Foito, Alexandre; Byrne, Stephen L.; Barth, Susanne] TEAGASC, Crops Environm & Land Use Programme, Oak Pk Res Ctr, Carlow, Ireland. [Foito, Alexandre; Stewart, Derek] James Hutton Inst, Enhancing Crop Prod & Utilisat, Dundee DD2 5DA, Scotland. [Hackett, Christine Anne] Biomath & Stat Scotland, Dundee DD2 5DA, Scotland. [Byrne, Stephen L.] Aarhus Univ, Dept Mol Biol & Genet, Res Ctr Flakkebjerg, DK-4200 Slagelse, Denmark. RP Barth, S (reprint author), TEAGASC, Crops Environm & Land Use Programme, Oak Pk Res Ctr, Carlow, Ireland. EM susanne.barth@teagasc.ie OI Byrne, Stephen/0000-0002-1179-2272 FU Irish Department of Agriculture, Fisheries and Marine [RSF 06-346] FX We are grateful to the expert help in manually editing metabolite data to Alexandre Gervaise. This study was financed through a Research Stimulus Fund Grant by the Irish Department of Agriculture, Fisheries and Marine (RSF 06-346). NR 59 TC 1 Z9 1 U1 0 U2 17 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1573-3882 EI 1573-3890 J9 METABOLOMICS JI Metabolomics PD APR PY 2015 VL 11 IS 2 BP 412 EP 424 DI 10.1007/s11306-014-0703-5 PG 13 WC Endocrinology & Metabolism SC Endocrinology & Metabolism GA CC7TC UT WOS:000350570300016 ER PT J AU Woodruff, DR Meinzer, FC Marias, DE Sevanto, S Jenkins, MW McDowell, NG AF Woodruff, David R. Meinzer, Frederick C. Marias, Danielle E. Sevanto, Sanna Jenkins, Michael W. McDowell, Nate G. TI Linking nonstructural carbohydrate dynamics to gas exchange and leaf hydraulic behavior in Pinus edulis and Juniperus monosperma SO NEW PHYTOLOGIST LA English DT Article DE carbon starvation; carbon storage; drought; growth limitation; Juniperus monosperma; leaf hydraulics; nonstructural carbohydrate (NSC); Pinus edulis ID WATER-STRESS; STOMATAL CONDUCTANCE; PHLOEM TRANSPORT; TREE MORTALITY; DROUGHT STRESS; DOUGLAS-FIR; DIE-OFF; CARBON; FOREST; PLANTS AB Leaf hydraulics, gas exchange and carbon storage in Pinus edulis and Juniperus monosperma, two tree species on opposite ends of the isohydry-anisohydry spectrum, were analyzed to examine relationships between hydraulic function and carbohydrate dynamics. Leaf hydraulic vulnerability, leaf water potential ((l)), leaf hydraulic conductance (K-leaf), photosynthesis (A), stomatal conductance (g(s)) and nonstructural carbohydrate (NSC) content were analyzed throughout the growing season. Leaf hydraulic vulnerability was significantly lower in the relatively anisohydric J.monosperma than in the more isohydric P.edulis. In P.edulis, (l) dropped and stayed below 50% loss of leaf hydraulic conductance (P-50) early in the day during May, August and around midday in September, leading to sustained reductions in K-leaf. In J.monosperma, (l) dropped below P-50 only during August, resulting in the maintenance of K-leaf during much of the growing season. Mean A and g(s) during September were significantly lower in P.edulis than in J.monosperma. Foliar total NSC was two to three times greater in J.monosperma than in P.edulis in June, August and September. Consistently lower levels of total NSC in P.edulis suggest that its isohydric strategy pushes it towards the exhaustion of carbon reserves during much of the growing season. C1 [Woodruff, David R.; Meinzer, Frederick C.] US Forest Serv, USDA, PNW Res Stn, Corvallis, OR 97331 USA. [Marias, Danielle E.] Oregon State Univ, Coll Forestry, Corvallis, OR 97331 USA. [Sevanto, Sanna; McDowell, Nate G.] Los Alamos Natl Lab, Earth & Environm Sci Div, Los Alamos, NM 87545 USA. [Jenkins, Michael W.] Univ Calif Santa Cruz, Dept Environm Studies, Santa Cruz, CA 95064 USA. RP Woodruff, DR (reprint author), US Forest Serv, USDA, PNW Res Stn, 3200 SW Jefferson Way, Corvallis, OR 97331 USA. EM dwoodruff@fs.fed.us FU Los Alamos National Laboratory [DE-NA0001302]; USDA Forest Service Pacific Northwest Research Station [DE-NA0001302]; Department of Energy, Office of Science FX This work was supported in part by interagency agreement DE-NA0001302 between Los Alamos National Laboratory and the USDA Forest Service Pacific Northwest Research Station, and by the Department of Energy, Office of Science. We are grateful to Kristen Falk for help with laboratory work and to three anonymous reviewers for comments that resulted in an improved paper. NR 54 TC 10 Z9 11 U1 13 U2 74 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0028-646X EI 1469-8137 J9 NEW PHYTOL JI New Phytol. PD APR PY 2015 VL 206 IS 1 BP 411 EP 421 DI 10.1111/nph.13170 PG 11 WC Plant Sciences SC Plant Sciences GA CC4TT UT WOS:000350347500039 PM 25412472 ER PT J AU Tao, Y Wang, FT Jia, DM Li, JT Zhang, YM Jia, CG Wang, DP Pan, HY AF Tao, Ye Wang, Fengting Jia, Dongmei Li, Jingtao Zhang, Yamei Jia, Chengguo Wang, Dongping Pan, Hongyu TI Cloning and Functional Analysis of the Promoter of a Stress-inducible Gene (ZmRXO1) in Maize SO PLANT MOLECULAR BIOLOGY REPORTER LA English DT Article DE Maize; Stress-inducible; Promoter cloning; Functional analysis ID ARABIDOPSIS-THALIANA; REGULATORY ELEMENTS; EXPRESSION; PLANTS; TRANSDUCTION; RESISTANCE; SEQUENCES; PROTEIN; POTATO AB The ZmRXO1 gene is a nucleotide-binding site leucine-rich repeat (NBS-LRR) type of R gene in maize (Zea mays). To understand the regulatory mechanism of ZmRXO1 gene expression, we isolated and characterized the ZmRXO1 promoter (PZmRXO1)-the 5' flanking region of ZmRXO1. A series of PZmRXO1 deletion derivatives, R1-R4, from the translation start code (-1,576, -934, -829, and -582) were fused to the GUS reporter gene, and each deletion construct was analyzed by Agrobacterium-mediated transformation into tobacco. Sequence analysis showed that several cis-acting elements (MBS, Box-I, TGA-element and CCAAT-box) were located within the promoter. Deletion analysis of the promoter suggested that the 1,576-bp fragment upstream of ZmRXO1 gene showed a high level of GUS expression in tobacco. The promoter sequence (-582 to -1) was sufficient to improve transcription of GUS gene under hormones (MeJA, GA, ABA), drought and low temperature. Moreover, there might be repressor elements in the region (-1,576 to -934 bp) to repress ZmRXO1 gene expression under treatment with salicylic acid. C1 [Tao, Ye; Wang, Fengting; Jia, Dongmei; Li, Jingtao; Zhang, Yamei; Jia, Chengguo; Pan, Hongyu] Jilin Univ, Coll Plant Sci, Changchun 130062, Jilin Province, Peoples R China. [Wang, Dongping] Los Alamos Natl Lab, Biosci Div, Los Alamos, NM 87544 USA. RP Pan, HY (reprint author), Jilin Univ, Coll Plant Sci, 5333 Xian Rd, Changchun 130062, Jilin Province, Peoples R China. EM panhongyu@jlu.edu.cn FU Twelfth Five Year Plan Project of Science and Technology Support, P.R. China [2012BAD19B04, 2014BAD14B02]; Ministry of Agriculture Key Project of GM Cultivation of New Varieties, P.R. China [2013ZX08004004]; Project of International Collaboration Plan in Jilin Province [20100723]; Research and Development of Industrial Technology Special at Jilin Provincial Development and Reform Commission [2013C001] FX This research was funded by the Twelfth Five Year Plan Project of Science and Technology Support, P.R. China (2012BAD19B04, 2014BAD14B02), the Ministry of Agriculture Key Project of GM Cultivation of New Varieties, P.R. China (2013ZX08004004), the Project of International Collaboration Plan in Jilin Province (20100723) and the Research and Development of Industrial Technology Special at Jilin Provincial Development and Reform Commission (2013C001). NR 27 TC 2 Z9 3 U1 3 U2 24 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0735-9640 EI 1572-9818 J9 PLANT MOL BIOL REP JI Plant Mol. Biol. Rep. PD APR PY 2015 VL 33 IS 2 BP 200 EP 208 DI 10.1007/s11105-014-0741-1 PG 9 WC Biochemical Research Methods; Plant Sciences SC Biochemistry & Molecular Biology; Plant Sciences GA CC9CK UT WOS:000350665000003 ER PT J AU Du, Q Lehoucq, RB Tartakovsky, AM AF Du, Qiang Lehoucq, R. B. Tartakovsky, A. M. TI Integral approximations to classical diffusion and smoothed particle hydrodynamics SO COMPUTER METHODS IN APPLIED MECHANICS AND ENGINEERING LA English DT Article DE Smooth Particle Hydrodynamics; Classical diffusion; Nonlocal diffusion; Nonlocal operator; Nonlocal Neumann condition; Numerical approximation ID VOLUME-CONSTRAINED PROBLEMS; BOUNDARY-CONDITIONS; NONLOCAL DIFFUSION; PERIDYNAMIC STATES; EQUATIONS; NEUMANN; KERNEL; MODEL AB The contribution of the paper is the approximation of a classical diffusion operator by an integral equation with a volume constraint. A particular focus is on classical diffusion problems associated with Neumann boundary conditions. By exploiting this approximation, we can also approximate other quantities such as the flux out of a domain. Our analysis of the model equation on the continuum level is closely related to the recent work on nonlocal diffusion and peridynamic mechanics. In particular, we elucidate the role of a volumetric constraint as an approximation to a classical Neumann boundary condition in the presence of physical boundary. The volume-constrained integral equation then provides the basis for accurate and robust discretization methods. An immediate application is to the understanding and improvement of the Smoothed Particle Hydrodynamics (SPH) method. (C) 2014 Elsevier B.V. All rights reserved. C1 [Du, Qiang] Columbia Univ, Dept Appl Phys & Appl Math, New York, NY 10027 USA. [Du, Qiang] Penn State Univ, Dept Math, University Pk, PA 16802 USA. [Lehoucq, R. B.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Tartakovsky, A. M.] Univ S Florida, Dept Math & Stat, Sch Geosci, Tampa, FL 33620 USA. [Tartakovsky, A. M.] Pacific NW Natl Lab, Computat Math Grp, Richland, WA 99352 USA. RP Du, Q (reprint author), Columbia Univ, Dept Appl Phys & Appl Math, New York, NY 10027 USA. EM qd2125@columbia.edu; rblehou@sandia.gov; alexandre.tartakovsky@pnnl.gov RI Du, Qiang/B-1021-2008 OI Du, Qiang/0000-0002-1067-8937 FU US NSF [DMS-1318586]; AFOSR MURI center; US Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; US Department of Energy, Office of Science, Office of Advanced Scientific Computing Research, Applied Mathematics program; US Department of Energy [DE-AC05-76RL01830] FX Research of Q. Du was supported in part by US NSF DMS-1318586, and AFOSR MURI center for material failure prediction through peridynamics. Sandia is a multi-program laboratory managed and operated by Sandia Corporation, a wholly subsidiary of Lockheed Martin Corporation, for the US Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. A. Tartakovsky was supported by the US Department of Energy, Office of Science, Office of Advanced Scientific Computing Research, Applied Mathematics program. Pacific Northwest National Laboratory is operated by Battelle for the US Department of Energy under Contract DE-AC05-76RL01830. NR 31 TC 3 Z9 4 U1 1 U2 22 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0045-7825 EI 1879-2138 J9 COMPUT METHOD APPL M JI Comput. Meth. Appl. Mech. Eng. PD APR 1 PY 2015 VL 286 BP 216 EP 229 DI 10.1016/j.cma.2014.12.019 PG 14 WC Engineering, Multidisciplinary; Mathematics, Interdisciplinary Applications; Mechanics SC Engineering; Mathematics; Mechanics GA CB8DB UT WOS:000349857700011 ER PT J AU Travis, BJ Schubert, G AF Travis, B. J. Schubert, G. TI Keeping Enceladus warm SO ICARUS LA English DT Article DE Enceladus; Interiors; Thermal histories ID CHONDRITE PARENT BODIES; ICE SHELL; HEAT-FLUX; WATER; CONVECTION; EVOLUTION; DIFFERENTIATION; EUROPA; PLUME; FLOW AB Despite its small size, Enceladus emits considerable heat, especially at its south pole, even long after simple thermal models predict it should be frozen. Several sources of energy have been proposed as responsible for this heating, such as tidal dissipative heating (TDH), convection and shearing in the ice shell, and exothermic chemical reactions (e.g., serpentine formation). Crater relaxation simulations suggest that episodic heating events have occurred over long stretches of Enceladus' history. Thermal history and hydrothermal simulations reported here show that a combination of steady plus episodic TDH heating could maintain at least a polar ocean to the present time. Hydrothermal circulation can play a significant role in mining Enceladus' internal heat, facilitating the persistence of an ocean even to the present by focusing internal heat to the polar regions. Published by Elsevier Inc. C1 [Travis, B. J.] Los Alamos Natl Lab, Computat Earth Sci Grp, EES MS T003 16, Los Alamos, NM 87545 USA. [Travis, B. J.] Planetary Sci Inst, Tucson, AZ 85719 USA. [Schubert, G.] Univ Calif Los Angeles, Earth Planetary & Space Sci Dept, Los Angeles, CA 90095 USA. RP Travis, BJ (reprint author), Los Alamos Natl Lab, Computat Earth Sci Grp, EES MS T003 16, POB 1663, Los Alamos, NM 87545 USA. EM bjtravis@lanl.gov; schubert@ucla.edu FU Institute for Geophysics and Planetary Physics at Los Alamos National Laboratory; NASA Grant [NNH09AM58I] FX This work was supported by a grant from the Institute for Geophysics and Planetary Physics at Los Alamos National Laboratory and by NASA Grant NNH09AM58I: Thermal and Chemical Evolution of Icy Satellites. NR 52 TC 10 Z9 10 U1 8 U2 29 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0019-1035 EI 1090-2643 J9 ICARUS JI Icarus PD APR PY 2015 VL 250 BP 32 EP 42 DI 10.1016/j.icarus.2014.11.017 PG 11 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CB8KJ UT WOS:000349878200004 ER PT J AU Hawkins, CA Momen, MA Garvey, SL Kestell, J Kaminski, MD Dietz, ML AF Hawkins, Cory A. Momen, M. A. Garvey, Sarah L. Kestell, John Kaminski, Michael D. Dietz, Mark L. TI Evaluation of solid-supported room-temperature ionic liquids containing crown ethers as media for metal ion separation and preconcentration SO TALANTA LA English DT Article DE Extraction chromatography; Ionic liquids; Crown ethers; Strontium ID EXTRACTION CHROMATOGRAPHIC RESIN; ACIDIC NITRATE MEDIA; CYPHOS-IL-101 TETRADECYL(TRIHEXYL)PHOSPHONIUM CHLORIDE; MACROPOROUS RESINS; PARTITION CHROMATOGRAPHY; SOLVENT-EXTRACTION; CYPHOS IL-101; RARE-EARTHS; MACROCYCLE INTERACTION; BIOPOLYMER CAPSULES AB Extraction chromatographic (EXC) resins incorporating an appropriate crown ether in an oxygenated organic solvent such as 1-octanol are well established as sorbents for the analytical-scale separation and preconcentration of radiostrontium from a variety of sample types. Recent solvent extraction studies employing crown ethers in various 1-alkyl-3-methylimidazolium-based (C(n)C(1)im(+)) room-temperature ionic liquids (RTILs) indicate that under certain conditions, distribution ratios (D-sr) for strontium far in excess of those observed with conventional organic solvents are observed. To determine if this increase in liquid-liquid extraction efficiency will lead to improved strontium sorbents, several EXC resins and sol-gel glasses incorporating di-tert-butylcyclohexano-18-crown-6 (DtBuCH18C6) in either 1-decyl-3-methylimidazolium bis[(trifluoromethyl)sulfonyl]imide (C(10)C(1)imTf(2)N) or the related hydroxyalkyl-functionalized IL 1-(12-hydroxydodecyl)-3-butylimidazolium bis[trifluoromethyl)sulfonyllimide (C(12)OHC(4)im Tf2N) were prepared and characterized. Unexpectedly the performance of these materials was not uniformly better than that of a conventional EXC resin, an apparent result of the greater viscosity of the ionic liquids and the lower solubility of the crown ether in ILs versus conventional organic solvents. (C) 2014 Elsevier B.V. All rights reserved. C1 [Hawkins, Cory A.; Momen, M. A.; Garvey, Sarah L.; Kestell, John; Dietz, Mark L.] Univ Wisconsin, Dept Chem & Biochem, Milwaukee, WI 53211 USA. [Hawkins, Cory A.; Kaminski, Michael D.; Dietz, Mark L.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Dietz, ML (reprint author), Univ Wisconsin, Dept Chem & Biochem, 3210N Cramer St, Milwaukee, WI 53211 USA. EM dietzm@uwm.edu FU United States Department of Energy under the Single Investigator Small Group Research (SISGR) Program through sub-contract with Brookhaven National Laboratory (liquid-liquid extraction studies); PG Research Foundation [DtBuCH18C6]; Centers for Disease Control and Prevention [08FED894832]; National Center for Environmental Health, Division of Laboratory Sciences (sorbent characterization) FX The authors gratefully acknowledge the financial support of this work by the Office of Basic Energy Sciences of the United States Department of Energy under the Single Investigator Small Group Research (SISGR) Program through sub-contract with Brookhaven National Laboratory (liquid-liquid extraction studies); the PG Research Foundation (isolation of single isomeric forms of DtBuCH18C6); and the Centers for Disease Control and Prevention (Grant no. 08FED894832), National Center for Environmental Health, Division of Laboratory Sciences (sorbent characterization). NR 71 TC 5 Z9 5 U1 13 U2 84 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0039-9140 EI 1873-3573 J9 TALANTA JI Talanta PD APR 1 PY 2015 VL 135 BP 115 EP 123 DI 10.1016/j.talanta.2014.12.019 PG 9 WC Chemistry, Analytical SC Chemistry GA CB6IM UT WOS:000349730700017 PM 25640134 ER PT J AU de Juan, F Politano, A Chiarello, G Fertig, HA AF de Juan, Fernando Politano, Antonio Chiarello, Gennaro Fertig, Herbert A. TI Symmetries and selection rules in the measurement of the phonon spectrum of graphene and related materials SO CARBON LA English DT Article ID INELASTIC ELECTRON-SCATTERING; METAL CARBIDE SURFACES; MONOLAYER GRAPHITE; DISPERSION; NI(111); INTERCALATION; BOND; SPECTROSCOPY; PT(111); PLASMON AB When the phonon spectrum of a material is measured in a scattering experiment, selection rules preclude the observation of phonons that are odd under reflection by the scattering plane. Understanding these rules is crucial to correctly interpret experiments and to detect broken symmetries. Taking graphene as a case study, in this work we derive the complete set of selection rules for the honeycomb lattice, showing that some of them have been missed or misinterpreted in the literature. Focusing on the technique of high-resolution electron energy loss spectroscopy (HREELS), we calculate the scattering intensity for a simple force constant model to illustrate these rules. In addition, we present HREELS measurements of the phonon dispersion for graphene on Ru(0001) and find excellent agreement with the theory. We also illustrate the effect of different symmetry breaking scenarios in the selection rules and discuss previous experiments in light of our results. Finally we clarify why the shear horizontal label is not equivalent to odd parity, and how this can be misleading in the identification of selection rules. (C) 2015 Elsevier Ltd. All rights reserved. C1 [de Juan, Fernando] Lawrence Berkeley Natl Labs, Div Mat Sci, Berkeley, CA 94720 USA. [de Juan, Fernando] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Politano, Antonio; Chiarello, Gennaro] Univ Calabria, Dipartmento Fis, I-87036 Arcavacata Di Rende, Cs, Italy. [Chiarello, Gennaro] Consorzio Nazl Interuniv Sci Fis Mat, I-00146 Rome, Italy. [Fertig, Herbert A.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. RP de Juan, F (reprint author), Lawrence Berkeley Natl Labs, Div Mat Sci, Berkeley, CA 94720 USA. EM ferdejuan@berkeley.edu RI de Juan, Fernando/B-9392-2008; OI de Juan, Fernando/0000-0001-6852-1484; CHIARELLO, Gennaro/0000-0002-3888-2980 FU "Programa Nacional de Movilidad de Recursos Humanos" (Spanish MECD); National Science Foundation (NSF) [DMR-1005035]; US-Israel Binational Science Foundation FX The authors would like to thank Davide Campi for helpful discussions. F. de J. acknowledges support from the "Programa Nacional de Movilidad de Recursos Humanos" (Spanish MECD). This work was supported in part by the National Science Foundation (NSF) through Grant No. DMR-1005035 and by the US-Israel Binational Science Foundation. NR 58 TC 10 Z9 10 U1 7 U2 25 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0008-6223 EI 1873-3891 J9 CARBON JI Carbon PD APR PY 2015 VL 85 BP 225 EP 232 DI 10.1016/j.carbon.2014.12.105 PG 8 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CB6GE UT WOS:000349724700025 ER PT J AU Ye, JC Charnvanichborikarn, S Worsley, MA Kucheyev, SO Wood, BC Wang, YM AF Ye, J. C. Charnvanichborikarn, S. Worsley, M. A. Kucheyev, S. O. Wood, B. C. Wang, Y. M. TI Enhanced electrochemical performance of ion-beam-treated 3D graphene aerogels for lithium ion batteries SO CARBON LA English DT Article ID MECHANICAL-PROPERTIES; LAYER GRAPHENE; SINGLE-LAYER; STORAGE; NETWORKS; NANOSHEETS; DEFECTS AB High energy light-ion (3.8 MeV He) bombardment is used to introduce lattice defects in a 3dimensional (3D) interconnected network of graphene aerogels (GAs). When these materials are used as anodes for lithium ion batteries, we observe improved percentage reversible capacity and cycle stability compared to those without ion-beam treatment. Furthermore, all ion-beam treated 3D graphene samples exhibit substantially higher Coulombic efficiencies, suggesting at beneficial role of vacancy-type defects in stabilizing solid-electrolyte interphases. Although 3D graphene exhibits initial reversible capacities that are 2-3 times higher than that of graphite (similar to 372 mAh/g), fast capacity fading is observed but becomes more stable after ion-beam treatment. Our experimental results demonstrate that ionbeam treatment is an effective route to tune and produce good-performance graphene electrodes, and that vacancy-type defects help to promote reversible lithium storage capacity in graphene. We further observe that 3D GAs irradiated to the highest dose studied (1016 cm(-2)) fail rapidly upon electrochemical cycling, likely caused by the excessive ion-beam damage and graphene restacking. Raman I(D)/I(D') signature is considered linked to defect type in graphene and thus is proposed, for the first time, as an indicator of the reversible capacity for GAs, (C) 2015 Elsevier Ltd. All rights reserved. C1 [Ye, J. C.; Charnvanichborikarn, S.; Worsley, M. A.; Kucheyev, S. O.; Wood, B. C.; Wang, Y. M.] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94550 USA. RP Wang, YM (reprint author), Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94550 USA. EM ymwang@llnl.gov RI Wang, Yinmin (Morris)/F-2249-2010; OI Worsley, Marcus/0000-0002-8012-7727 FU LLNL [DE-AC52-07NA27344]; Laboratory Directed Research and Development (LDRD) programs of LLNL [12-ERD-053, 15-ERD-022, 13-LW-099]; UC Lab Fees Research Program [12-LR-235323] FX The work was performed under the auspices of the US Department of Energy by LLNL under contract No. DE-AC52-07NA27344. The project was supported by the Laboratory Directed Research and Development (LDRD) programs of LLNL (12-ERD-053, 15-ERD-022, and 13-LW-099). The materials synthesis of this work was also supported by the UC Lab Fees Research Program under award 12-LR-235323. The authors wish to thank Drs. L.Y.L. Woo, A. Goldstein, and S. Shin for helpful discussion and TEM assistance. NR 28 TC 12 Z9 12 U1 3 U2 98 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0008-6223 EI 1873-3891 J9 CARBON JI Carbon PD APR PY 2015 VL 85 BP 269 EP 278 DI 10.1016/j.carbon.2014.12.097 PG 10 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CB6GE UT WOS:000349724700030 ER PT J AU Xue, Q Battistoni, M Powell, CF Longman, DE Quan, SP Pomraning, E Senecal, PK Schmidt, DP Som, S AF Xue, Q. Battistoni, M. Powell, C. F. Longman, D. E. Quan, S. P. Pomraning, E. Senecal, P. K. Schmidt, D. P. Som, S. TI An Eulerian CFD model and X-ray radiography for coupled nozzle flow and spray in internal combustion engines SO INTERNATIONAL JOURNAL OF MULTIPHASE FLOW LA English DT Article DE Computational fluid dynamics (CFD); Eulerian; Internal combustion engines (ICEs); Nozzle flow; Sprays; X-ray radiography ID DIESEL SPRAY; ATOMIZATION MODEL; SPATIAL ACCURACY; AMBIENT DENSITY; 2-PHASE FLOW; SIMULATIONS; INJECTORS; JETS; SOOT AB This paper implements a coupled approach to integrate the internal nozzle flow and the ensuing fuel spray using a Volume-of-Fluid (VOF) method in the finite-volume framework. A VOF method is used to model the internal nozzle two-phase flow with a cavitation description closed by the homogeneous relaxation model of Bilicki and Kestin (1990). An Eulerian single velocity field approach by Vallet et al. (2001) is implemented for near-nozzle spray modeling. This Eulerian approach considers the liquid and gas phases as a complex mixture with a highly variable density to describe near nozzle dense sprays. The liquid mass fraction is transported with a model for the turbulent liquid diffusion flux into the gas. Fully-coupled nozzle flow and spray simulations are performed in three dimensions and validated against the X-ray radiography measurements of Kastengren et al. (2014) for a diesel fuel surrogate. A standard k-epsilon Reynolds Averaged Navier Stokes based turbulence model is used in this study and the influence of model constants is evaluated. First, the grid convergence study is performed. The effect of grid size is also evaluated by comparing the fuel distribution against experimental data. Finally, the fuel distribution predicted by the coupled Eulerian approach is compared against that by Lagrangian-Eulerian spray model along with experimental data. The coupled Eulerian approach provides a unique way of coupling the nozzle flow and sprays so that the effects of in-nozzle flow can be directly realized on the fuel spray. Both experiment and numerical simulations show non-cavitation occurring for this injector with convergent nozzle geometry. The study shows that the Eulerian approach has advantages over near-field dense spray distributions. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Xue, Q.; Battistoni, M.; Powell, C. F.; Longman, D. E.; Som, S.] Argonne Natl Lab, Div Energy Syst, Argonne, IL 60439 USA. [Quan, S. P.; Pomraning, E.; Senecal, P. K.] Convergent Sci Inc, Middleton, WI 53562 USA. [Schmidt, D. P.] Univ Massachusetts, Dept Mech & Ind Engn, Amherst, MA 01002 USA. RP Xue, Q (reprint author), Argonne Natl Lab, Div Energy Syst, 9700 S Cass Ave, Argonne, IL 60439 USA. EM qxue@anl.gov RI Battistoni, Michele/M-9194-2014 OI Battistoni, Michele/0000-0001-6807-9657 FU DOEs Office of Vehicle Technologies, Office of Energy Efficiency and Renewable Energy; U.S. Department of Energy (DOE) [DE-AC02-06CH11357] FX This research was funded by DOEs Office of Vehicle Technologies, Office of Energy Efficiency and Renewable Energy. The authors wish to thank Gurpreet Singh and Leo Breton, team leader at DOE, for his support. This research was performed at the 7-BM and 32-ID beam lines of the APS at Argonne National Laboratory. Use of the APS is supported by the U.S. Department of Energy (DOE) under Contract No. DE-AC02-06CH11357. NR 75 TC 17 Z9 17 U1 5 U2 40 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0301-9322 EI 1879-3533 J9 INT J MULTIPHAS FLOW JI Int. J. Multiph. Flow PD APR PY 2015 VL 70 BP 77 EP 88 DI 10.1016/j.ijmultiphaseflow.2014.11.012 PG 12 WC Mechanics SC Mechanics GA CB4BR UT WOS:000349573700006 ER PT J AU Huang, L Idir, M Zuo, C Kaznatcheev, K Zhou, L Asundi, A AF Huang, Lei Idir, Mourad Zuo, Chao Kaznatcheev, Konstantine Zhou, Lin Asundi, Anand TI Shape reconstruction from gradient data in an arbitrarily-shaped aperture by iterative discrete cosine transforms in Southwell configuration SO OPTICS AND LASERS IN ENGINEERING LA English DT Article DE Shape reconstruction from gradient; Wavefront reconstruction; Arbitrarily-shaped aperture; Discrete cosine transform; Southwell configuration ID WAVE-FRONT RECONSTRUCTION; DIFFERENCE MEASUREMENTS; FRINGE REFLECTOMETRY; FOURIER-TRANSFORMS; OPTICAL TEST; INTEGRATION; SURFACES AB The shape reconstruction from gradient data is a common problem in many slope-based metrology applications. In practice, the gradient data may not be ideally available for the whole field of view as expected, due to the aperture or the unmeasurable part of sample. An iterative method by using discrete cosine transforms is addressed in this work to deal with the integration problem with incomplete gradient dataset in Southwell configuration. Simulation indicates that the discrete cosine transform provides better initial values than discrete Fourier transform does, and it converges to a more accurate level by updating with spectrum-based slopes comparing to the slope updates from finite difference in classical method. Experimental results show the feasibility of the proposed approach in a practical measurement. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Huang, Lei; Idir, Mourad; Kaznatcheev, Konstantine; Zhou, Lin] Brookhaven Natl Lab, NSLS 2, Upton, NY 11973 USA. [Kaznatcheev, Konstantine] Nanjing Univ Sci & Technol, Jiangsu Key Lab Spectral Imaging & Intelligence S, Nanjing 210094, Jiangsu, Peoples R China. [Kaznatcheev, Konstantine; Zhou, Lin] Natl Univ Def Technol, Coll Mechatron Engn & Automat, Changsha 410073, Hunan, Peoples R China. [Kaznatcheev, Konstantine; Asundi, Anand] Nanyang Technol Univ, Sch Mech & Aerosp Engn, Singapore 639798, Singapore. RP Huang, L (reprint author), Brookhaven Natl Lab, NSLS 2, 50 Rutherford Dr, Upton, NY 11973 USA. EM huanglei0114@gmail.com RI Zuo, Chao/D-7273-2014; OI Zuo, Chao/0000-0002-1461-0032; Asundi, Anand/0000-0003-3835-4624 NR 24 TC 4 Z9 4 U1 3 U2 13 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0143-8166 EI 1873-0302 J9 OPT LASER ENG JI Opt. Lasers Eng. PD APR PY 2015 VL 67 BP 176 EP 181 DI 10.1016/j.optlaseng.2014.11.011 PG 6 WC Optics SC Optics GA CB4EO UT WOS:000349581200020 ER PT J AU Liu, F Lin, L Vigil-Fowler, D Lischner, J Kemper, AF Sharifzadeh, S da Jornadad, FH Deslippe, J Yang, C Neaton, JB Louie, SG AF Liu, Fang Lin, Lin Vigil-Fowler, Derek Lischner, Johannes Kemper, Alexander F. Sharifzadeh, Sahar da Jornadad, Felipe H. Deslippe, Jack Yang, Chao Neaton, Jeffrey B. Louie, Steven G. TI Numerical integration for ab initio many-electron self energy calculations within the GW approximation SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE GW; Self energy; Convolution; Numerical integration; Trapezoidal rule; Principal value integration; COHSEX; XCOR; Dyson's equation ID QUASI-PARTICLE; GREENS-FUNCTION; DENSITY; MATRIX; SOLIDS; GAS AB We present a numerical integration scheme for evaluating the convolution of a Green's function with a screened Coulomb potential on the real axis in the GW approximation of the self energy. Our scheme takes the zero broadening limit in Green's function first, replaces the numerator of the integrand with a piecewise polynomial approximation, and performs principal value integration on subintervals analytically. We give the error bound of our numerical integration scheme and show by numerical examples that it is more reliable and accurate than the standard quadrature rules such as the composite trapezoidal rule. We also discuss the benefit of using different self energy expressions to perform the numerical convolution at different frequencies. (C) 2015 Elsevier Inc. All rights reserved. C1 [Liu, Fang] Cent Univ Finance & Econ, Sch Math & Stat, Beijing 100081, Peoples R China. [Lin, Lin] Univ Calif Berkeley, Dept Math, Berkeley, CA 94720 USA. [Lin, Lin; Kemper, Alexander F.; Yang, Chao] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, Berkeley, CA 94720 USA. [Vigil-Fowler, Derek; Lischner, Johannes; da Jornadad, Felipe H.; Neaton, Jeffrey B.; Louie, Steven G.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Sharifzadeh, Sahar] Boston Univ, Dept Elect & Comp Engn, Boston, MA 02215 USA. [Sharifzadeh, Sahar] Boston Univ, Div Engn & Mat Sci, Boston, MA 02215 USA. [Deslippe, Jack] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, NERSC, Berkeley, CA 94720 USA. [Vigil-Fowler, Derek; Lischner, Johannes; da Jornadad, Felipe H.; Neaton, Jeffrey B.; Louie, Steven G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Neaton, Jeffrey B.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. RP Liu, F (reprint author), Cent Univ Finance & Econ, Sch Math & Stat, Beijing 100081, Peoples R China. EM fliu@lsec.cc.ac.cn; linlin@math.berkeley.edu; vigil@berkeley.edu; jlischner597@gmail.com; afkemper@lbl.gov; ssharifz@bu.edu; jornada@berkeley.edu; jdeslippe@lbl.gov; cyang@lbl.gov; jbneaton@lbl.gov; sglouie@berkeley.edu RI Neaton, Jeffrey/F-8578-2015; Foundry, Molecular/G-9968-2014; Kemper, Alexander/F-8243-2016; Sharifzadeh, Sahar/P-4881-2016 OI Neaton, Jeffrey/0000-0001-7585-6135; Kemper, Alexander/0000-0002-5426-5181; Sharifzadeh, Sahar/0000-0003-4215-4668 FU Scientific Discovery through Advanced Computing (SciDAC) program on Excited State Phenomena in Energy Materials - U.S. Department of Energy, Office of Science; Basic Energy Sciences Program [DE-AC02-05CH11231]; Office of Advanced Scientific Computing Research of the U. S. Department of Energy [DE-AC02-05CH11232]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; National Science Foundation of China [11071265, 11171232]; Foundation for University Key Teacher by the China Scholarship Council; Central University of Finance and Economics; Laboratory Directed Research and Development Program of Lawrence Berkeley National Laboratory under the U. S. Department of Energy [DE-AC02-05CH11231]; Simons Foundation Fellowship in Theoretical Physics; Advanced Scientific Computing Research Program FX Partial support for this work was provided through Scientific Discovery through Advanced Computing (SciDAC) program on Excited State Phenomena in Energy Materials funded by U.S. Department of Energy, Office of Science, the Advanced Scientific Computing Research Program and the Basic Energy Sciences Program under contract number DE-AC02-05CH11231 at the Lawrence Berkeley National Laboratory. The computational results were obtained at the National Energy Research Scientific Computing Center (NERSC), which is supported by the Director, Office of Advanced Scientific Computing Research of the U.S. Department of Energy under contract number DE-AC02-05CH11232. Work at the Molecular Foundry was supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under contract number DE-AC02-05CH11231. F.L. is also grateful to the support from the National Science Foundation of China (grants 11071265 and 11171232), and the Foundation for University Key Teacher by the China Scholarship Council and the Central University of Finance and Economics. This work was completed during her visit to Lawrence Berkeley National Laboratory. L. L. and A. F. K. also acknowledge the support by the Laboratory Directed Research and Development Program of Lawrence Berkeley National Laboratory under the U. S. Department of Energy contract number DE-AC02-05CH11231. S. G. L. acknowledges the support of a Simons Foundation Fellowship in Theoretical Physics. NR 26 TC 2 Z9 2 U1 0 U2 15 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD APR 1 PY 2015 VL 286 BP 1 EP 13 DI 10.1016/j.jcp.2015.01.023 PG 13 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA CB4MA UT WOS:000349600600001 ER PT J AU Philip, B Berrill, MA Allu, S Hamilton, SP Sampath, RS Clarno, KT Dilts, GA AF Philip, Bobby Berrill, Mark A. Allu, Srikanth Hamilton, Steven P. Sampath, Rahul S. Clarno, Kevin T. Dilts, Gary A. TI A parallel multi-domain solution methodology applied to nonlinear thermal transport problems in nuclear fuel pins SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Inexact Newton; Jacobian free Newton Krylov; Krylov subspace method; Domain decomposition; Preconditioning; Iterative method; Parallel algorithm ID INEXACT NEWTON METHODS; HEAT-TRANSFER; DE-NOVO; SYSTEMS; CODE AB This paper describes an efficient and nonlinearly consistent parallel solution methodology for solving coupled nonlinear thermal transport problems that occur in nuclear reactor applications over hundreds of individual 3D physical subdomains. Efficiency is obtained by leveraging knowledge of the physical domains, the physics on individual domains, and the couplings between them for preconditioning within a Jacobian Free Newton Krylov method. Details of the computational infrastructure that enabled this work, namely the open source Advanced Multi-Physics (AMP) package developed by the authors is described. Details of verification and validation experiments, and parallel performance analysis in weak and strong scaling studies demonstrating the achieved efficiency of the algorithm are presented. Furthermore, numerical experiments demonstrate that the preconditioner developed is independent of the number of fuel subdomains in a fuel rod, which is particularly important when simulating different types of fuel rods. Finally, we demonstrate the power of the coupling methodology by considering problems with couplings between surface and volume physics and coupling of nonlinear thermal transport in fuel rods to an external radiation transport code. (C) 2015 Elsevier Inc. All rights reserved. C1 [Philip, Bobby; Berrill, Mark A.; Allu, Srikanth; Hamilton, Steven P.; Sampath, Rahul S.; Clarno, Kevin T.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Dilts, Gary A.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Philip, B (reprint author), Oak Ridge Natl Lab, One Bethel Valley Rd, Oak Ridge, TN 37831 USA. EM philipb@ornl.gov OI Philip, Bobby/0000-0001-6716-3515; Clarno, Kevin/0000-0002-5999-2978; Berrill, Mark/0000-0002-4525-3939; allu, srikanth/0000-0003-2841-4398 FU Nuclear Energy Advanced Modeling and Simulation (NEAMS) program of the U.S. Department of Energy Office of Nuclear Energy, Advanced Modeling and Simulation Office; U.S. Department of Energy, Office of Science, Office of Advanced Scientific Computing Research, Applied Mathematics program, Extreme Scale Solvers project (EASIR); Office of Science of the U.S. Department of Energy [DE-AC05-00OR22725]; Eugene P. Wigner Fellowship at Oak Ridge National Laboratory; U.S. Department of Energy [DE-AC05-00OR22725] FX The AMP (Advanced Multi-Physics) code is distributed with a modified BSD license and accessible either by contacting the corresponding author or through the Radiation Safety Information Computational Center (RSICC) at Oak Ridge National Laboratory, with an RSICC license, as CCC-793. The development of AMP, and the nuclear fuel performance application built upon it, was funded by the Nuclear Energy Advanced Modeling and Simulation (NEAMS) program of the U.S. Department of Energy Office of Nuclear Energy, Advanced Modeling and Simulation Office. This material is also based upon work supported by the U.S. Department of Energy, Office of Science, Office of Advanced Scientific Computing Research, Applied Mathematics program, Extreme Scale Solvers project (EASIR).; This research used resources of the Oak Ridge Leadership Computing Facility at the Oak Ridge National Laboratory, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC05-00OR22725. Mark Berrill acknowledges support from the Eugene P. Wigner Fellowship at Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy under Contract DE-AC05-00OR22725. NR 37 TC 3 Z9 3 U1 1 U2 7 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD APR 1 PY 2015 VL 286 BP 143 EP 171 DI 10.1016/j.jcp.2015.01.029 PG 29 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA CB4MA UT WOS:000349600600011 ER PT J AU Koleske, DD Fischer, AJ Bryant, BN Kotula, PG Wierer, JJ AF Koleske, D. D. Fischer, A. J. Bryant, B. N. Kotula, P. G. Wierer, J. J. TI On the increased efficiency in InGaN-based multiple quantum wells emitting at 530-590 nm with AlGaN interlayers SO JOURNAL OF CRYSTAL GROWTH LA English DT Article DE Interfaces; X-ray diffraction; Metalorganic vapor phase epitaxy; InGaN; Light-emitting diodes; Solar cells ID TRANSMISSION ELECTRON-MICROSCOPY; X-RAY-DIFFRACTION; INDIUM INCORPORATION; GALLIUM NITRIDE; GAN; DIODES; DISLOCATIONS; HYDROGEN; GREEN; FLUCTUATIONS AB InGaN/AlGaN/GaN-based multiple quantum wells (MQWs) with AlGaN inLerlayers (lLs) are investigated, specifically to examine the fundamental mechanisms behind their increased radiative efficiency at wavelengths 01 530-590 nm. The AlzGa1-zN (z similar to 0.38) IL is similar to 1-2 nm thick, and is grown after and at the same growth temperature as the 3 rim thick InGaN quantum well (QW). This is followed by an increase in temperature for the growth of a 10 nm thick GaN barrier layer. The insertion of the AlGaN IL within the MQW provides various benefits. First, the AlGaN IL allows for growth of the InxGa1-xN QW well below typical growth temperatures to achieve higher x (up to similar to 0.25). Second, annealing the IL capped QW prior to the GaN barrier growth improves the AlGaN IL smoothness as determined by atomic force microscopy, improves the InGaN/AIGaN/GaN interface quality as determined from scanning transmission electron microscope images and x-ray diffraction, and increases the radiative efficiency by reducing non-radiative defects as determined by Lime-resolved photoluminescence measurements. Finally, the AlGaN IL increases the spontaneous and piezoelectric polarization induced electric fields acting on the InGaN QW, providing an additional red-shift to the emission wavelength as determined by Schrodinger-Poisson modeling and fitting to the experimental data. The relative impact of increased indium concentration and polarization fields on the radiative efficiency of MQWs with AlGaN ILs is explored along with implications to conventional longer wavelength emitters. (C) 2015 Elsevier By. All rights reserved. C1 [Koleske, D. D.; Fischer, A. J.; Kotula, P. G.; Wierer, J. J.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Bryant, B. N.] Univ New Mexico, Ctr High Technol Mat, Albuquerque, NM 87131 USA. RP Koleske, DD (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM ddkoles@sandia.gov RI Kotula, Paul/A-7657-2011; Wierer, Jonathan/G-1594-2013 OI Kotula, Paul/0000-0002-7521-2759; Wierer, Jonathan/0000-0001-6971-4835 FU Sandia's Solid-State Lighting Science Energy Frontier Research Center - US Department of Energy, Office of Basic Energy Sciences; MQWs growth; LDRD program at Sandia National Laboratories; Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX J.M. Kempisty is thanked for technical assistance and K.C. Cross for AFM measurements. The single-QW annealing work was supported by the Sandia's Solid-State Lighting Science Energy Frontier Research Center, funded by the US Department of Energy, Office of Basic Energy Sciences and the MQWs growth and characterization was supported by the LDRD program at Sandia National Laboratories, Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Company, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 49 TC 3 Z9 3 U1 1 U2 78 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-0248 EI 1873-5002 J9 J CRYST GROWTH JI J. Cryst. Growth PD APR 1 PY 2015 VL 415 BP 57 EP 64 DI 10.1016/j.jcrysgro.2014.12.034 PG 8 WC Crystallography; Materials Science, Multidisciplinary; Physics, Applied SC Crystallography; Materials Science; Physics GA CB4NC UT WOS:000349603500011 ER PT J AU Gorichok, IV Fochuk, PM Verzhak, YV Parashchuk, TO Freik, DM Panchuk, OE Bolotnikov, AE James, RB AF Gorichok, I. V. Fochuk, P. M. Verzhak, Ye. V. Parashchuk, T. O. Freik, D. M. Panchuk, O. E. Bolotnikov, A. E. James, R. B. TI Compensation mechanism of bromine dopants in cadmium telluride single crystals SO JOURNAL OF CRYSTAL GROWTH LA English DT Article DE Computer simulation; Point defects; Bridgman technique; Semiconducting cadmium compounds ID SELF-COMPENSATION; CDTE; DEFECTS; IDENTIFICATION; DONOR AB Cadmium telluride single crystals, doped by Bromine, were grown by Bridgman method and annealed under cadmium overpressure (P-cd=10(2) - 10(5) Pa) at 800-1100 K. Their electrical properties at high- and low temperature have been investigated. The influence of impurities on the crystal electrical properties has been analyzed by using the defective subsystem model, which includes the possibility of formation of point intrinsic (V-cd(2-), Cd-i(2+,) V-Te(2+,) Te-i(2-)) and replacement defects (Br-Te(0), Br-Te(+)), and also point defects complexes (Br-Te(+) V-cd(2-)), (2Br(Te)(+) V-cd(-))(0). It was established that the concentration dependence between free charge carriers and annealing process parameters (n(T), n(P-cd)) are determined by two dominant defects-Br-Te(+) and (2Br(Te)(+) V-cd(2-)). Their content varies with the annealing temperature and the vapor pressure of the component; the concentration of other defects is much smaller and almost does not influence the electron density. (C) 2014 Elsevier B.V. All rights reserved. C1 [Gorichok, I. V.; Parashchuk, T. O.; Freik, D. M.] Vasyl Stefanyk Precarpathian Natl Univ, Phys Chem Inst, Ivano Frankivsk, Ukraine. [Fochuk, P. M.; Verzhak, Ye. V.; Panchuk, O. E.] Yuriy Fedkovych Chernivtsi Natl Univ, Dept Inorg Chem, Chernovtsy, Ukraine. [Bolotnikov, A. E.; James, R. B.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Gorichok, IV (reprint author), Vasyl Stefanyk Precarpathian Natl Univ, Phys Chem Inst, Ivano Frankivsk, Ukraine. EM horichokihor@gmail.com RI Fochuk, Petro/D-9409-2016; Panchuk, Oleg/C-1764-2017 OI Fochuk, Petro/0000-0002-4149-4882; Panchuk, Oleg/0000-0003-3906-1858 FU Science@Technology Center of Ukraine [P406]; DOE/NNSA DNN R@D; U.S. Department of Energy FX This work was partly supported by the Science@Technology Center of Ukraine under Project P406 with the U.S. Department of Energy and by DOE/NNSA DNN R@D. NR 35 TC 5 Z9 5 U1 7 U2 22 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-0248 EI 1873-5002 J9 J CRYST GROWTH JI J. Cryst. Growth PD APR 1 PY 2015 VL 415 BP 146 EP 151 DI 10.1016/j.jcrysgro.2014.11.005 PG 6 WC Crystallography; Materials Science, Multidisciplinary; Physics, Applied SC Crystallography; Materials Science; Physics GA CB4NC UT WOS:000349603500025 ER PT J AU Tooker, BC Brindley, SM Chiarappa-Zucca, ML Turteltaub, KW Newman, LS AF Tooker, Brian C. Brindley, Stephen M. Chiarappa-Zucca, Marina L. Turteltaub, Kenneth W. Newman, Lee S. TI Accelerator mass spectrometry detection of beryllium ions in the antigen processing and presentation pathway SO JOURNAL OF IMMUNOTOXICOLOGY LA English DT Article DE Accelerator mass spectrometry (AMS); beryllium; chronic beryllium disease; metal antigen; metal processing ID CD4(+) T-CELLS; HLA-DP; PROLIFERATIVE RESPONSE; DISEASE; LYMPHOCYTES; FREQUENCY; EXPOSURE; BLOOD; RISK AB Exposure to small amounts of beryllium (Be) can result in beryllium sensitization and progression to Chronic Beryllium Disease (CBD). In CBD, beryllium is presented to Be-responsive T-cells by professional antigen-presenting cells (APC). This presentation drives T-cell proliferation and pro-inflammatory cytokine (IL-2, TNF alpha, and IFN gamma) production and leads to granuloma formation. The mechanism by which beryllium enters an APC and is processed to become part of the beryllium antigen complex has not yet been elucidated. Developing techniques for beryllium detection with enough sensitivity has presented a barrier to further investigation. The objective of this study was to demonstrate that Accelerator Mass Spectrometry (AMS) is sensitive enough to quantify the amount of beryllium presented by APC to stimulate Be-responsive T-cells. To achieve this goal, APC - which may or may not stimulate Be-responsive T-cells - were cultured with Be-ferritin. Then, by utilizing AMS, the amount of beryllium processed for presentation was determined. Further, IFN gamma intracellular cytokine assays were performed to demonstrate that Be-ferritin (at levels used in the experiments) could stimulate Be-responsive T-cells when presented by an APC of the correct HLA type (HLA-DP0201). The results indicated that Be-responsive T-cells expressed IFN gamma only when APC with the correct HLA type were able to process Be for presentation. Utilizing AMS, it was determined that APC with HLA-DP0201 had membrane fractions containing 0.17-0.59 ng Be and APC with HLA-DP0401 had membrane fractions bearing 0.40-0.45 ng Be. However, HLA-DP0401 APC had 20-times more Be associated with the whole cells (57.68-61.12 ng) than HLA-DP0201 APC (0.90-3.49 ng). As these findings demonstrate, AMS detection of picogram levels of Be processed by APC is possible. Further, regardless of form, Be requires processing by APC to successfully stimulate Be-responsive T-cells to generate IFN gamma. C1 [Tooker, Brian C.; Brindley, Stephen M.; Newman, Lee S.] Univ Colorado Denver, Dept Med, Sch Med, Div Allergy & Clin Immunol, Aurora, CO 80045 USA. [Chiarappa-Zucca, Marina L.] Div Chem Sci, Livermore, CA USA. [Turteltaub, Kenneth W.] Lawrence Livermore Natl Lab, Biosci & Biotechnol Div, Livermore, CA USA. RP Tooker, BC (reprint author), Univ Colorado Denver, Ctr Worker Hlth & Environm, Dept Environm & Occupat Hlth, Colorado Sch Publ Hlth, Bldg RC2,Room 10420D,Mail Stop B164,12700 E 19th, Aurora, CO 80045 USA. EM brian.tooker@ucdenver.edu OI Tooker, Brian/0000-0002-0018-3658 FU NIEHS NIH HHS [P01 ES011810]; NIGMS NIH HHS [P41 GM103483] NR 22 TC 0 Z9 0 U1 0 U2 7 PU INFORMA HEALTHCARE PI NEW YORK PA 52 VANDERBILT AVE, NEW YORK, NY 10017 USA SN 1547-691X EI 1547-6901 J9 J IMMUNOTOXICOL JI J. Immunotoxicol. PD APR-JUN PY 2015 VL 12 IS 2 BP 181 EP 187 DI 10.3109/1547691X.2014.917748 PG 7 WC Toxicology SC Toxicology GA CB1RG UT WOS:000349405100011 PM 24932923 ER PT J AU Tarditi, AM Imhoff, C Braun, F Miller, JB Gellman, AJ Cornaglia, L AF Tarditi, Ana M. Imhoff, Carolina Braun, Fernando Miller, James B. Gellman, Andrew J. Cornaglia, Laura TI PdCuAu ternary alloy membranes: Hydrogen permeation properties in the presence of H2S SO JOURNAL OF MEMBRANE SCIENCE LA English DT Article DE PdCuAu ternary alloy; Hydrogen separation; Sulfur tolerance ID COMPOSITE MEMBRANES; PALLADIUM; PERFORMANCE; SEPARATION; PD; PERMEABILITY; METHANE; SULFIDE; BINARY; PD/CU AB PdCuAu ternary alloy membranes with different component compositions were synthesized by sequential electroless deposition of components onto porous stainless steel substrates. The ternary with the highest Au content, Pd69Cu14Au17, exhibited the highest hydrogen permeation flux, comparable to that of a Pd91Au9 membrane. Upon exposure to 100 ppm H2S/H-2 at 673 K for 24 h, all PdCuAu membranes experienced flux reductions of similar to 55%, followed by recovery to similar to 80% of the initial hydrogen flux upon reintroduction of pure hydrogen at 400 degrees C. Complete flux recovery after H2S exposure required hydrogen treatment at 500 degrees C. X-ray diffraction (XRD) analysis of the H2S-exposed PdCuAu membranes revealed fcc alloy structure with no evidence of bulk sulfide formation. In agreement with the XRD results, sulfur was not defected in the bulk of H2S-exposed samples by energy dispersive spectroscopy (EDS). However, analysis of H2S-exposed PdCuAu alloys by X-ray photoelectron spectroscopy (XPS) depth profiling revealed low, but measureable, amounts of sulfur in the near surface region, about 10 nm in depth. The depth profiles of samples after hydrogen recovery treatment showed significantly reduced sulfur content. These results indicate that H2S exposure causes flux loss in PdCuAu alloys through a surface-poisoning mechanism, and that the surface sulfide can be removed-and flux recovered-by high temperature treatment in hydrogen. (C) 2014 Elsevier B.V. All rights reserved. C1 [Tarditi, Ana M.; Imhoff, Carolina; Braun, Fernando; Cornaglia, Laura] UNL CONICET, Inst Invest Catalisis & Petroquim FIQ, RA-3000 Santa Fe, Argentina. [Miller, James B.; Gellman, Andrew J.] Carnegie Mellon Univ, Dept Chem Engn, Pittsburgh, PA 15213 USA. [Miller, James B.; Gellman, Andrew J.] US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15262 USA. RP Tarditi, AM (reprint author), UNL CONICET, Inst Invest Catalisis & Petroquim FIQ, Santiago del Estero 2829, RA-3000 Santa Fe, Argentina. EM atarditi@fiq.unl.edu.ar RI Gellman, Andrew/M-2487-2014 OI Gellman, Andrew/0000-0001-6618-7427 FU UNL [CAID 2012 PJ50020110100052LI]; ANPCyT [PIP 2012-00955]; NSF-CONICET Program [2011-2013]; National Science Foundation [CBET 1033804] FX The authors wish to acknowledge the financial support received from UNL (CAID 2012 PJ50020110100052LI), ANPCyT (PIP 2012-00955) and the NSF-CONICET Program (Grant 2011-2013). Thanks are given to Elsa Grimaldi for the English language editing, The authors also wish to acknowledge the National Science Foundation for its support of research on Pd-alloys for hydrogen separation at Carnegie Mellon (CBET 1033804). NR 27 TC 8 Z9 8 U1 2 U2 35 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0376-7388 EI 1873-3123 J9 J MEMBRANE SCI JI J. Membr. Sci. PD APR 1 PY 2015 VL 479 BP 246 EP 255 DI 10.1016/j.memsci.2014.12.030 PG 10 WC Engineering, Chemical; Polymer Science SC Engineering; Polymer Science GA CB4TB UT WOS:000349620000028 ER PT J AU Dane, M Gonis, A Nicholson, DM Stocks, GM AF Daene, M. Gonis, A. Nicholson, D. M. Stocks, G. M. TI Solving the self-interaction problem in Kohn-Sham density functional theory: Application to atoms SO JOURNAL OF PHYSICS AND CHEMISTRY OF SOLIDS LA English DT Article DE Ab initio calculations; Electronic structure ID APPROXIMATION AB In previous work, we proposed a computational methodology that addresses the elimination of the self-interaction error from the Kohn-Sham formulation of the density functional theory. We demonstrated how the exchange potential can be obtained, and presented results of calculations for atomic systems up to Kr carried out within a Cartesian coordinate system. In this paper, we provide complete details of this self-interaction free method formulated in spherical coordinates based on the explicit equidensity basis ansatz. We prove analytically that derivatives obtained using this method satisfy the Virial theorem for spherical orbitals, where the problem can be reduced to one dimension. We present the results of calculations of ground-state energies of atomic systems throughout the periodic table carried out within the exchange-only mode. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Daene, M.; Gonis, A.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Nicholson, D. M.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. [Stocks, G. M.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Dane, M (reprint author), Lawrence Livermore Natl Lab, POB 808,L-372, Livermore, CA 94551 USA. EM daene1@llnl.gov RI Stocks, George Malcollm/Q-1251-2016 OI Stocks, George Malcollm/0000-0002-9013-260X FU U.S. DOE [DE-AC52-07NA27344]; LLNS, LLC; Division of Materials Sciences and Engineering, Office of Basic Energy Sciences; Center for Defect Physics in Structural Materials; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences FX The work at LLNL is supported by the U.S. DOE under Contract DE-AC52-07NA27344 with LLNS, LLC (MD, AG). Research at ORNL is sponsored by the Division of Materials Sciences and Engineering, Office of Basic Energy Sciences (DMN, GMS), and the Center for Defect Physics in Structural Materials (CDP), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences (DMN, GMS). NR 14 TC 2 Z9 2 U1 1 U2 13 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0022-3697 EI 1879-2553 J9 J PHYS CHEM SOLIDS JI J. Phys. Chem. Solids PD APR PY 2015 VL 79 BP 55 EP 65 DI 10.1016/j.jpcs.2014.09.013 PG 11 WC Chemistry, Multidisciplinary; Physics, Condensed Matter SC Chemistry; Physics GA CB3CE UT WOS:000349505000007 ER PT J AU Amsbaugh, JF Barrett, J Beglarian, A Bergmann, T Bichsel, H Bodine, LI Bonn, J Boyd, NM Burritt, TH Chaoui, Z Chilingaryan, S Corona, TJ Doe, PJ Dunmore, JA Enomoto, S Formaggio, JA Frankle, FM Furse, D Gemmeke, H Gluck, F Harms, F Harper, GC Hartmann, J Howe, MA Kaboth, A Kelsey, J Knauer, M Kopmann, A Leber, ML Martin, EL Middleman, KJ Myers, AW Oblath, NS Parno, DS Peterson, DA Petzold, L Phillips, DG Renschler, P Robertson, RGH Schwarz, J Steidl, M Tcherniakhovski, D Thummler, T Van Wechel, TD VanDevender, BA Vocking, S Wall, BL Wierman, KL Wilkerson, JF Wustling, S AF Amsbaugh, J. F. Barrett, J. Beglarian, A. Bergmann, T. Bichsel, H. Bodine, L. I. Bonn, J. Boyd, N. M. Burritt, T. H. Chaoui, Z. Chilingaryan, S. Corona, T. J. Doe, P. J. Dunmore, J. A. Enomoto, S. Formaggio, J. A. Fraenkle, F. M. Furse, D. Gemmeke, H. Glueck, F. Harms, F. Harper, G. C. Hartmann, J. Howe, M. A. Kaboth, A. Kelsey, J. Knauer, M. Kopmann, A. Leber, M. L. Martin, E. L. Middleman, K. J. Myers, A. W. Oblath, N. S. Parno, D. S. Peterson, D. A. Petzold, L. Phillips, D. G., II Renschler, P. Robertson, R. G. H. Schwarz, J. Steidl, M. Tcherniakhovski, D. Thuemmler, T. Van Wechel, T. D. VanDevender, B. A. Voecking, S. Wall, B. L. Wierman, K. L. Wilkerson, J. F. Wuestling, S. TI Focal-plane detector system for the KATRIN experiment SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Neutrino mass; Low-background counting; Si p-i-n diode; Vacuum; Data acquisition ID TRITIUM BETA-DECAY; NEUTRINO MASS; HIGH-RESOLUTION; SEARCH; FIELD; SPECTROMETER; ELECTRONS; ARRAY AB The local plane detector system for the KArlsiuhe TRItium Neutrino (KATRIN) experiment consists of a multi-pixel silicon p-i-n-diode array, custom readout electronics, two superconducting solenoid magnets, an ultra high vacuum system, a high vacuum system, calibration and monitoring devices, a scintillating veto, and a custom data-acquisition system, It is designed to detect the low-energy electrons selected by the KATRIN main spectrometer. We describe the system and summarize its performance after its final installation. (C) 2015 Elsevier B.V. All rights reserved. C1 [Amsbaugh, J. F.; Bichsel, H.; Bodine, L. I.; Boyd, N. M.; Burritt, T. H.; Doe, P. J.; Dunmore, J. A.; Enomoto, S.; Harper, G. C.; Leber, M. L.; Martin, E. L.; Myers, A. W.; Parno, D. S.; Peterson, D. A.; Robertson, R. G. H.; Van Wechel, T. D.; VanDevender, B. A.; Wall, B. L.; Wierman, K. L.] Univ Washington, Ctr Expt Nucl Phys & Astrophys, Dept Phys, Seattle, WA 98195 USA. [Barrett, J.; Formaggio, J. A.; Furse, D.; Kaboth, A.; Kelsey, J.; Oblath, N. S.] MIT, Nucl Sci Lab, Cambridge, MA 02139 USA. [Beglarian, A.; Bergmann, T.; Chilingaryan, S.; Gemmeke, H.; Hartmann, J.; Kopmann, A.; Petzold, L.; Tcherniakhovski, D.; Wuestling, S.] Karlsruhe Inst Technol, Inst Data Proc & Elect, D-76344 Eggenstein Leopoldshafen, Germany. [Bonn, J.] Johannes Gutenberg Univ Mainz, Inst Phys, D-55099 Mainz, Germany. [Chaoui, Z.] Univ Setif, Lab Optoelect & Devices, Setif 19000, Algeria. [Corona, T. J.; Fraenkle, F. M.; Howe, M. A.; Phillips, D. G., II; Wierman, K. L.; Wilkerson, J. F.] Univ N Carolina, Dept Phys, Chapel Hill, NC 27599 USA. [Corona, T. J.; Fraenkle, F. M.; Howe, M. A.; Phillips, D. G., II; Wierman, K. L.; Wilkerson, J. F.] Triangle Univ Nucl Lab, Durham, NC 27708 USA. [Glueck, F.; Harms, F.; Renschler, P.; Schwarz, J.] Karlsruhe Inst Technol, Inst Expt Nucl Phys, D-76344 Eggenstein Leopoldshafen, Germany. [Glueck, F.] Wigner Res Ctr Phys, H-1525 Budapest, Hungary. [Knauer, M.; Steidl, M.; Thuemmler, T.] Karlsruhe Inst Technol, Inst Nucl Phys, D-76344 Eggenstein Leopoldshafen, Germany. [Middleman, K. J.] STFC Daresbury Lab, ASTeC Vacuum Sci Grp, Warrington WA4 4AD, Cheshire, England. [Voecking, S.] Univ Munster, Inst Nucl Phys, D-48149 Munster, Germany. [Wilkerson, J. F.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Parno, DS (reprint author), Univ Washington, Ctr Expt Nucl Phys & Astrophys, Dept Phys, Seattle, WA 98195 USA. EM dparno@uw.edu RI Kopmann, Andreas/B-3454-2013; chaoui, zine el abidine/P-7018-2016; Parno, Diana/B-7546-2017; OI Kopmann, Andreas/0000-0002-2362-3943; chaoui, zine el abidine/0000-0001-7452-3515; Parno, Diana/0000-0002-9363-0401; Bodine, Laura/0000-0002-2926-8479 FU U.S. Department of Energy Office of Science, Office of Nuclear Physics [DE-FG02-97ER41020, DE-FG02-97ER41041, FG02-97ER41033]; German Helmholtz Gemeinschaft and Bundesministerium fur Bildung und Forschung; Karlsruhe House of Young Scientists FX This material is based upon work supported by the U.S. Department of Energy Office of Science, Office of Nuclear Physics under Award Number DE-FG02-97ER41020, which provided primary support for construction, and under Award Numbers DE-FG02-97ER41041 and DE-FG02-97ER41033. The electronics subsystem has been provided through grants from the German Helmholtz Gemeinschaft and Bundesministerium fur Bildung und Forschung. Some travel support was provided by the Karlsruhe House of Young Scientists. The active interest of Canberra Industries in meeting our specialized requirements is appreciated. We gratefully acknowledge the participation, interest, and strong support of the entire KATRIN collaboration. NR 56 TC 5 Z9 5 U1 0 U2 8 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD APR 1 PY 2015 VL 778 BP 40 EP 60 DI 10.1016/j.nima.2014.12.116 PG 21 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CB2PC UT WOS:000349468900007 ER PT J AU Cherepy, NJ Sanner, RD Beck, PR Swanberg, EL Tillotson, TM Payne, SA Hurlbut, CR AF Cherepy, Nerine J. Sanner, Robert D. Beck, Patrick R. Swanberg, Erik L. Tillotson, Thomas M. Payne, Stephen A. Hurlbut, Charles R. TI Bismuth- and lithium-loaded plastic scintillators for gamma and neutron detection SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Plastic scintillator; Gamma plastic; Neutron plastic; Neutron capture scintillator; Phoswich; Pulse-shape discrimination ID PULSE-SHAPE DISCRIMINATION; ORGANIC SCINTILLATORS; SPECTROSCOPY; RADIATION AB Transparent plastic scintillators based on polyvinyltoluene (PVT) have been fabricated with high loading of bismuth carboxylates for gamma spectroscopy, and with lithium carboxylates for neutron detection. When activated with a combination of standard fluors, 2,5-diphenyloxazole (PPO) and tetraphenylbutadiene (TPB), gamma light yields with 15 wt% bismuth tripivalate of 5000 Ph/MeV are measured. A PVT plastic formulation including 30 wt% lithium pivalate and 30 wt% PPO offers both pulse shape discrimination, and a neutron capture peak at similar to 400 keVee. In another configuration, a bismuth-loaded PVT. plastic is coated with ZnS(Li-6) paint, permitting simultaneous gamma and neutron detection via pulse shape discrimination with a figure-of-merit of 3.8, while offering gamma spectroscopy with energy resolution of R(662 keV)=15%. (C) 2015 Elsevier B.V. All rights reserved. C1 [Cherepy, Nerine J.; Sanner, Robert D.; Beck, Patrick R.; Swanberg, Erik L.; Tillotson, Thomas M.; Payne, Stephen A.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Hurlbut, Charles R.] Eljen Technol, Sweetwater, TX USA. RP Cherepy, NJ (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. EM cherepy1@llnl.gov RI Cherepy, Nerine/F-6176-2013 OI Cherepy, Nerine/0000-0001-8561-923X FU National Nuclear Security Administration, Defense Nuclear Nonproliferation Research and Development Office of the U.S. Department of Energy [DE-AC03-76SF00098]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344, LLNL-JRNL-663264] FX This work was supported by the National Nuclear Security Administration, Defense Nuclear Nonproliferation Research and Development Office of the U.S. Department of Energy under Contract DE-AC03-76SF00098, and was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344, Release number LLNL-JRNL-663264. NR 22 TC 8 Z9 8 U1 3 U2 30 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD APR 1 PY 2015 VL 778 BP 126 EP 132 DI 10.1016/j.nima.2015.01.008 PG 7 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CB2PC UT WOS:000349468900017 ER PT J AU Roni, MS Jin, MZ Eksioglu, SD AF Roni, Mohammad S. Jin, Mingzhou Eksioglu, Sandra D. TI A hybrid inventory management system responding to regular demand and surge demand SO OMEGA-INTERNATIONAL JOURNAL OF MANAGEMENT SCIENCE LA English DT Article DE Hybrid inventory policy; Surge demand; Level Crossing Theory; Mixed integer programming ID SERVICE LEVEL CONSTRAINTS; RATIONING POLICY; LOST-SALES; EMERGENCY ORDERS; DISRUPTION RISKS; COSTS; MODEL; SUPPLIERS; SINGLE; TIME AB This paper proposes a hybrid policy for a stochastic inventory system facing regular demand and surge demand. The combination of two different demand patterns can be observed in many areas, such as healthcare inventory and humanitarian supply chain management. The surge demand has a lower arrival rate but higher demand volume per arrival. The solution approach proposed in this paper incorporates the level crossing method and mixed integer programming technique to optimize the hybrid inventory policy with both regular orders and emergency orders. The level crossing method is applied to obtain the equilibrium distributions of inventory levels under a given policy. The model is further transformed into a mixed integer program to identify an optimal hybrid policy. A sensitivity analysis is conducted to investigate the impact of parameters on the optimal inventory policy and minimum cost. Numerical results clearly show the benefit of using the proposed hybrid inventory model. The model and solution approach could help healthcare providers or humanitarian logistics providers in managing their emergency supplies in responding to surge demands. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Roni, Mohammad S.] Idaho Natl Lab, Idaho Falls, ID 83402 USA. [Jin, Mingzhou] Univ Tennessee, Dept Ind & Syst Engn, Knoxville, TN 37996 USA. [Eksioglu, Sandra D.] Clemson Univ, Dept Ind Engn, Clemson, SC 29631 USA. RP Jin, MZ (reprint author), Univ Tennessee, Dept Ind & Syst Engn, 525D John Tickle Engn Bldg,851 Neyland Dr, Knoxville, TN 37996 USA. EM jin@utk.edu; seksiog@clemson.edu RI Eksioglu, Sandra/G-8623-2016 OI Eksioglu, Sandra/0000-0002-6674-2133 NR 53 TC 2 Z9 2 U1 5 U2 51 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0305-0483 J9 OMEGA-INT J MANAGE S JI Omega-Int. J. Manage. Sci. PD APR PY 2015 VL 52 BP 190 EP 200 DI 10.1016/j.omega.2014.05.002 PG 11 WC Management; Operations Research & Management Science SC Business & Economics; Operations Research & Management Science GA CB4GS UT WOS:000349586800017 ER PT J AU Theuamaran, R Meshot, ER Daraio, C AF Theuamaran, Ramathasan Meshot, Eric R. Daraio, Chiara TI Shock formation and rate effects in impacted carbon nanotube foams SO CARBON LA English DT Article ID MECHANICAL-PROPERTIES; ENERGY-DISSIPATION; IN-SITU; AEROGELS; ARRAYS; COMPRESSION; BUNDLES AB We investigate rate-effects in the dynamic response of vertically aligned carbon nanotube (VACNT) foams excited by impacts at controlled velocities. They exhibit a complex rate-dependent loading-unloading response at low impact velocities and they support shock formation beyond a critical velocity. The measured critical velocities are similar to 10 times lower than in other foams of similar densities a desirable characteristic in impact protective applications. In-situ high-speed microscopy reveals strain localization and progressive buckling at low velocities and a crush-front propagation during shock compression. We correlate these responses to quantitative measurements of the density gradient and fiber morphology, obtained with spatially resolved X-ray scattering and mass attenuation. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Theuamaran, Ramathasan; Daraio, Chiara] CALTECH, Div Engn & Appl Sci, Pasadena, CA 91125 USA. [Theuamaran, Ramathasan; Daraio, Chiara] Swiss Fed Inst Technol, Dept Mech & Proc Engn, Swiss Fed Inst Technol Zurich, CH-8092 Zurich, Switzerland. [Meshot, Eric R.] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94551 USA. RP Daraio, C (reprint author), Swiss Fed Inst Technol, Dept Mech & Proc Engn, Swiss Fed Inst Technol Zurich, CH-8092 Zurich, Switzerland. EM daraio@ethz.ch RI Daraio, Chiara/N-2170-2015 OI Daraio, Chiara/0000-0001-5296-4440 FU Institute for Collaborative Biotechnologies (ICB) [W911NF-09-D-0001]; Army Research Office (ARO); U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Director, Office of Science, and Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-ACO2-05CH11231] FX We thank Ludovica Lattanzi and Wei-Hsun Lin for assistance in preparing the educational video, Jan Rys (ETH Zurich) and Darwin Zwissler (UC Berkeley, USA) for assistance during experiments. We acknowledge financial support from the Institute for Collaborative Biotechnologies (ICB) under the contract W911NF-09-D-0001 with the Army Research Office (ARO). A portion of this work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. Xray characterization was performed at beamline 7.3.3 at the Advanced Light Source, which is supported by the Director, Office of Science, and Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-ACO2-05CH11231. NR 41 TC 6 Z9 6 U1 5 U2 27 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0008-6223 EI 1873-3891 J9 CARBON JI Carbon PD APR PY 2015 VL 84 BP 390 EP 398 DI 10.1016/j.carbon.2014.12.006 PG 9 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CA5NQ UT WOS:000348955500044 ER PT J AU Zhang, C Ramirez-Marquez, JE Wang, JH AF Zhang, Chi Emmanuel Ramirez-Marquez, Jose Wang, Jianhui TI Critical infrastructure protection using secrecy - A discrete simultaneous game SO EUROPEAN JOURNAL OF OPERATIONAL RESEARCH LA English DT Article DE Critical infrastructure protection; Simultaneous game; Intentional attack; Information; Secrecy ID RESOURCE-ALLOCATION; PARALLEL SYSTEMS; DEFENSE STRATEGY; RELIABILITY; SECURITY; EQUILIBRIUM; PERFORMANCE; COMPONENTS; DECEPTION; ATTACKERS AB In this research, critical infrastructure protection against intentional attacks is modeled as a discrete simultaneous game between the protector and the attacker, to model the situation that both players keep the information of their resource allocation secret. We prove that keeping the information regarding protection strategies secret can obtain a better effect of critical infrastructure protection than truthfully disclosing it. Solving a game theoretic problem, even in the case of two players, has been known to be intractable. To deal with this complexity, after proving that pure-strategy Nash equilibrium solutions do not exist for the proposed simultaneous game, a new approach is proposed to identify its mixed-strategy Nash equilibrium solution. (C) 2014 Elsevier B.V. All rights reserved. C1 [Zhang, Chi] Tsinghua Univ, Dept Ind Engn, Beijing 100084, Peoples R China. [Emmanuel Ramirez-Marquez, Jose] Stevens Inst Technol, Sch Syst & Enterprises, Hoboken, NJ 07030 USA. [Wang, Jianhui] Argonne Natl Lab, Decis & Informat Sci Div, Argonne, IL 60439 USA. [Emmanuel Ramirez-Marquez, Jose] Tecnol Monterrey, Grad Sch, Guadalajara 45201, Jalisco, Mexico. RP Ramirez-Marquez, JE (reprint author), Stevens Inst Technol, Sch Syst & Enterprises, Hoboken, NJ 07030 USA. EM Jose.Ramirez-Marquez@stevens.edu RI zhang, chi/E-1251-2016 OI zhang, chi/0000-0002-2995-7469 FU National Natural Science Foundation of China [71301085, 71332005] FX The authors gratefully acknowledge the support from the National Natural Science Foundation of China under Grants 71301085 and 71332005. We also appreciate the effort and comments of Editor Immanuel Bomze and the anonymous referees that made the paper stronger. NR 42 TC 3 Z9 3 U1 3 U2 21 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0377-2217 EI 1872-6860 J9 EUR J OPER RES JI Eur. J. Oper. Res. PD APR 1 PY 2015 VL 242 IS 1 BP 212 EP 221 DI 10.1016/j.ejor.2014.10.001 PG 10 WC Management; Operations Research & Management Science SC Business & Economics; Operations Research & Management Science GA CA1QY UT WOS:000348687900020 ER PT J AU Zhou, XW Ward, DK Foster, M Zimmerman, JA AF Zhou, X. W. Ward, D. K. Foster, M. Zimmerman, J. A. TI An analytical bond-order potential for the copper-hydrogen binary system SO JOURNAL OF MATERIALS SCIENCE LA English DT Article ID EMBEDDED-ATOM-METHOD; AUSTENITIC STAINLESS-STEELS; FCC METALS; MULTICOMPONENT SYSTEMS; MOLECULAR-DYNAMICS; ALLOYS; CU; NI; EMBRITTLEMENT; OPTIMIZATION AB Despite extensive studies in the past, deterioration of mechanical properties due to hydrogen environment exposure remains a serious problem for structural materials. More effective improvement of a material's resilience requires advanced computational methods to elucidate the fundamental mechanisms of the hydrogen effects. To enable accurate molecular dynamics (MD) studies of the hydrogen effects on metals, we have developed a high-fidelity analytical bond-order potential (BOP) for the copper-hydrogen binary system as a representative case. This potential is available through the publically available MD code LAMMPS. The potential parameters are optimized using an iterative process. First, the potential is fitted to static and reactive properties of a variety of elemental and binary configurations including small clusters and bulk lattices (with coordination varying from 1 to 12). Then the potential is put through a series of rigorous MD simulation tests (e.g., vapor deposition and solidification) that involve chaotic initial configurations. It is demonstrated that this Cu-H BOP not only gives structural and property trends close to those seen in experiments and quantum mechanical calculations, but also predicts the correct phase transformations and chemical reactions in direct MD simulations. The correct structural evolution from chaotic initial states strongly verifies the transferability of the potential. A highly transferable potential is the reason that a well-parameterized analytical BOP can enable MD simulations of metal-hydrogen interactions to reach a fidelity level not achieved in the past. C1 [Zhou, X. W.; Zimmerman, J. A.] Sandia Natl Labs, Mech Mat Dept, Livermore, CA 94550 USA. [Ward, D. K.] Sandia Natl Labs, Radiat & Nucl Detect Mat & Anal Dept, Livermore, CA 94550 USA. [Foster, M.] Sandia Natl Labs, Dept Chem Mat, Livermore, CA 94550 USA. RP Zhou, XW (reprint author), Sandia Natl Labs, Mech Mat Dept, Livermore, CA 94550 USA. EM xzhou@sandia.gov FU US Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the US Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. This work was performed under a Laboratory Directed Research and Development (LDRD) project. NR 56 TC 2 Z9 2 U1 3 U2 27 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0022-2461 EI 1573-4803 J9 J MATER SCI JI J. Mater. Sci. PD APR PY 2015 VL 50 IS 7 BP 2859 EP 2875 DI 10.1007/s10853-015-8848-9 PG 17 WC Materials Science, Multidisciplinary SC Materials Science GA CB0MY UT WOS:000349321600004 ER PT J AU Jung, J Onen, A Russell, K Broadwater, RP Steffel, S Dinkel, A AF Jung, Jaesung Onen, Ahmet Russell, Kevin Broadwater, Robert P. Steffel, Steve Dinkel, Alex TI Configurable, Hierarchical, Model-based, Scheduling Control with photovoltaic generators in power distribution circuits SO RENEWABLE ENERGY LA English DT Article DE Reactive power control; Hierarchical control; Local control; Power distribution control; PV integration; Aggregation PV ID VOLTAGE RISE MITIGATION; LOAD RESEARCH DATA; COORDINATED CONTROL; DISTRIBUTION-SYSTEMS; ENERGY-STORAGE; PENETRATION; MICROGRIDS; OPERATION; STRATEGY; FLOW AB Existing distribution systems and their associated controls have been around for decades. Most distribution circuits have capacity to accommodate some level of PV generation, but the question is how much can they handle without creating problems. This paper proposes a Configurable, Hierarchical, Model-based, Scheduling Control (CHMSC) of automated utility control devices and photovoltaic (PV) generators. In the study here the automated control devices are assumed to be owned by the utility and the PV generators and PV generator controls by another party. The CHMSC, which exists in a hierarchical control architecture that is failure tolerant, strives to maintain the voltage level that existed before introducing the PV into the circuit while minimizing the circuit loss and reducing the motion of the automated control devices. This is accomplished using prioritized objectives. The CHMSC sends control signals to the local controllers of the automated control devices and PV controllers. To evaluate the performance of the CHMSC, increasing PV levels of adoption are analyzed in a model of an actual circuit that has significant existing PV penetration and automated voltage control devices. The CHMSC control performance is compared with that of existing, local control. Simulation results presented demonstrate that the CHMSC algorithm results in better voltage control, lower losses, and reduced automated control device motion, especially as the penetration level of PV increases. Published by Elsevier Ltd. C1 [Jung, Jaesung] Brookhaven Natl Lab, Sustainable Energy Technol Dept, Upton, NY 11973 USA. [Onen, Ahmet] Abdullah Gul Univ, Dept Elect & Elect Engn, Kayseri, Turkey. [Russell, Kevin] Elect Distribut Design Inc, Blacksburg, VA USA. [Broadwater, Robert P.] Virginia Polytech Inst & State Univ, Dept Elect & Comp Engn, Blacksburg, VA 24061 USA. [Steffel, Steve; Dinkel, Alex] Pepco Holdings Inc, Washington, DC USA. RP Jung, J (reprint author), Brookhaven Natl Lab, Sustainable Energy Technol Dept, Bldg 1798,POB 5000, Upton, NY 11973 USA. EM jsjung@bnl.gov RI Onen, Ahmet/N-6632-2014; OI Onen, Ahmet/0000-0001-7086-5112 FU Pepco Holdings, Inc.; Electrical Distribution Design, Inc. FX The authors would like to thank Pepco Holdings, Inc. and Electrical Distribution Design, Inc. for providing data, funding, and technical assistance used in this study. NR 29 TC 2 Z9 2 U1 0 U2 6 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0960-1481 J9 RENEW ENERG JI Renew. Energy PD APR PY 2015 VL 76 BP 318 EP 329 DI 10.1016/j.renene.2014.11.046 PG 12 WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Energy & Fuels SC Science & Technology - Other Topics; Energy & Fuels GA CA5NP UT WOS:000348955400035 ER PT J AU Kumagai, A Wu, L Iwamoto, S Lee, SH Endo, T Rodriguez, M Mielenz, JR AF Kumagai, Akio Wu, Long Iwamoto, Shinichiro Lee, Seung-Hwan Endo, Takashi Rodriguez, Miguel, Jr. Mielenz, Jonathan R. TI Improvement of enzymatic saccharification of Populus and switchgrass by combined pretreatment with steam and wet disk milling SO RENEWABLE ENERGY LA English DT Article DE Hot-compressed water; Wet disk milling; Populus; Switchgrass; Biorefinery ID BIOMASS RECALCITRANCE; CORN STOVER; RICE STRAW; CELL-WALL; LIGNOCELLULOSIC BIOMASS; SULFURIC-ACID; POPLAR; HYDROLYSIS; WATER; HEMICELLULOSES AB To reduce the recalcitrance of lignocellulosic biomass for subsequent biological processing, we pretreated energy crop feedstocks with mild steam treatment (ST; 130 and 150 degrees C for 60 min) and wet disk milling (WDM). We tested two phylogenetically different, but typical energy crop feedstocks: Populus trichocarpa and switchgrass (Panicum virgatum). WDM after ST facilitated the fibrillation of both types of biomass, resulting in an increase of specific surface area, improved enzymatic saccharification yield, and decrease in cellulose crystallinity. After steam treatment at 150 degrees C followed by 17 cycles of WDM, enzymatic hydrolysis resulted in almost complete glucan to glucose conversion in both feedstocks. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Kumagai, Akio; Wu, Long; Iwamoto, Shinichiro; Lee, Seung-Hwan; Endo, Takashi] Natl Inst Adv Ind Sci & Technol, Biomass Refinery Res Ctr, Hiroshima 7370046, Japan. [Lee, Seung-Hwan] Kangwon Natl Univ, Dept Forest Biomat Engn, Coll Forest & Environm Sci, Chunchon 200701, South Korea. [Rodriguez, Miguel, Jr.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. [Mielenz, Jonathan R.] Oak Ridge Natl Lab, BioEnergy Sci Ctr, Oak Ridge, TN 37831 USA. RP Endo, T (reprint author), Natl Inst Adv Ind Sci & Technol, Biomass Refinery Res Ctr, 3-11-32 Kagamiyama, Hiroshima 7370046, Japan. EM t-endo@aist.go.jp; biofuels4me@gmail.com RI Kumagai, Akio/L-5649-2016 OI Kumagai, Akio/0000-0002-5185-2145 FU Japan-U.S. cooperation project for research and standardization of Clean Energy Technologies FX This work was supported by the Japan-U.S. cooperation project for research and standardization of Clean Energy Technologies. NR 44 TC 1 Z9 1 U1 3 U2 15 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0960-1481 J9 RENEW ENERG JI Renew. Energy PD APR PY 2015 VL 76 BP 782 EP 789 DI 10.1016/j.renene.2014.11.070 PG 8 WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Energy & Fuels SC Science & Technology - Other Topics; Energy & Fuels GA CA5NP UT WOS:000348955400081 ER PT J AU Hale, LM Lim, H Zimmerman, JA Battaile, CC Weinberger, CR AF Hale, Lucas M. Lim, Hojun Zimmerman, Jonathan A. Battaile, Corbett C. Weinberger, Christopher R. TI Insights on activation enthalpy for non-Schmid slip in body-centered cubic metals SO SCRIPTA MATERIALIA LA English DT Article DE Dislocations; Slip; bcc metals; Iron ID NON-GLIDE STRESSES; SCREW DISLOCATIONS; PLASTIC-DEFORMATION; ANISOTROPIC ELASTICITY; COMPUTER-SIMULATION; CORE STRUCTURE; BCC METALS; MOLYBDENUM; MOTION; TEMPERATURE AB We use insights gained from atomistic simulation to develop an activation enthalpy model for dislocation slip in body-centered cubic iron. Using a classical potential that predicts dislocation core stabilities consistent with ab initio predictions, we quantify the non-Schmid stress-dependent effects of slip. The kink-pair activation enthalpy is evaluated and a model is identified as a function of the general stress state. Our model enlarges the applicability of the classic Kocks activation enthalpy model to materials with non-Schmid behavior. (C) 2014 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Hale, Lucas M.; Zimmerman, Jonathan A.] Sandia Natl Labs, Dept Mech Mat, Livermore, CA 94551 USA. [Lim, Hojun; Battaile, Corbett C.] Sandia Natl Labs, Dept Computat Mat & Data Sci, Albuquerque, NM 87185 USA. [Weinberger, Christopher R.] Drexel Univ, Dept Mech Engn & Mech, Philadelphia, PA 19104 USA. RP Hale, LM (reprint author), NIST, Thermodynam & Kinet Grp, Gaithersburg, MD 20899 USA. EM lmhale99@gmail.com FU Advanced Simulation and Computing - Physics and Engineering Models (ASC-P&EM) program at Sandia National Laboratories; United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work is supported by the Advanced Simulation and Computing - Physics and Engineering Models (ASC-P&EM) program at Sandia National Laboratories. Sandia is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed-Martin Corporation, for the United States Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 28 TC 3 Z9 3 U1 2 U2 22 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6462 J9 SCRIPTA MATER JI Scr. Mater. PD APR 1 PY 2015 VL 99 BP 89 EP 92 DI 10.1016/j.scriptamat.2014.11.035 PG 4 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA CA4NK UT WOS:000348881100023 ER PT J AU Remillieux, MC Anderson, BE Ulrich, TJ Le Bas, PY Payan, C AF Remillieux, Marcel C. Anderson, Brian E. Ulrich, T. J. Le Bas, Pierre-Yves Payan, Cedric TI Depth profile of a time-reversal focus in an elastic solid SO ULTRASONICS LA English DT Article DE Time-reversal; Elastodynamics; Lamb's problem ID ULTRASONIC FIELDS; WAVE SPECTROSCOPY; CHAOTIC CAVITIES; LOCALIZATION; PROPAGATION; SIMULATION; SURFACE AB The out-of-plane velocity component is focused on the flat surface of an isotropic solid sample using the principle of time reversal. This experiment is often reproduced in the context of nondestructive testing for imaging features near the surface of the sample. However, it is not clear how deep the focus extends into the bulk of the sample and what its profile is. In this paper, this question is answered using both numerical simulations and experimental data. The profiles of the foci are expressed in terms of the wavelengths of the dominant waves, based on the interpretation of the Lamb's problem and the use of the diffraction limit. Published by Elsevier B. V. C1 [Remillieux, Marcel C.; Anderson, Brian E.; Ulrich, T. J.; Le Bas, Pierre-Yves] Los Alamos Natl Lab, Geophys Grp EES 17, Los Alamos, NM 87545 USA. [Payan, Cedric] Aix Marseille Univ, Lab Mech & Acoust, LMA CNRS UPR 7051, F-13402 Marseille 20, France. RP Remillieux, MC (reprint author), Los Alamos Natl Lab, Geophys Grp EES 17, MS D446, Los Alamos, NM 87545 USA. EM mcr1@lanl.gov FU Los Alamos National Laboratory (LDRD program) FX We gratefully acknowledge the institutional support of the Los Alamos National Laboratory (LDRD program). NR 25 TC 1 Z9 1 U1 1 U2 15 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0041-624X EI 1874-9968 J9 ULTRASONICS JI Ultrasonics PD APR PY 2015 VL 58 BP 60 EP 66 DI 10.1016/j.ultras.2014.12.003 PG 7 WC Acoustics; Radiology, Nuclear Medicine & Medical Imaging SC Acoustics; Radiology, Nuclear Medicine & Medical Imaging GA CB1CX UT WOS:000349365400009 PM 25559066 ER PT J AU Abdo, AA Abeysekara, AU Alfaro, R Allen, BT Alvarez, C Alvarez, JD Arceo, R Arteaga-Velazquez, JC Aune, T Solares, HAA Barber, AS Baughman, BM Bautista-Elivar, N Gonzalez, JB Belmont, E BenZvi, SY Berley, D Rosales, MB Braun, J Caballero-Lopez, RA Caballero-Mora, KS Carraminiana, A Castillo, M Christopher, GE Cotti, U Cotzomi, J De la Fuente, E De Leon, C DeYoung, T Hernandez, RD Diaz-Cruz, KL Diaz-Velezi, JC Dingus, BL DuVernoisi, MA Ellsworth, RW Fiorinoi, D Fraija, N Galindo, A Garfias, F Gonzalez, MM Goodman, JA Grabski, V Gussert, M Hampel-Arias, Z Harding, JP Hays, E Hoffman, CM Hui, CM Huintemeyer, P Imrani, A Iriarte, A Kam, P Kieda, D Kolterman, BE Kunde, G Lara, A Lauer, R Lee, WH Lennarz, D Vargas, HL Linares, EC Linnemann, JT Longo, M Luna-Garcla, R MacGibbon, JH Marinelli, A Marinelli, SS Martinez, H Martinez, O Martinez-Castro, J Matthews, JAJ McEnery, J Torres, EM Mincer, AI Miranda-Romagnoli, P Moreno, E Morgan, T Mostafa, M Nellen, L Nemethy, P Newbold, M Noriega-Papaqui, R Oceguera-Becerra, T Patricelli, B Pelayo, R Perez-Perez, EG Pretz, J Riviere, C Rosa-Gonzalez, D Ruiz-Velasco, E Ryan, J Salazar, H Salesa, F Sandoval, A Parkinson, PMS Schneider, M Silich, S Sinnis, G Smith, AJ Stump, D Woodle, KS Springer, RW Taboada, I Toale, PA Tollefson, K Torres, I Ukwatta, TN Vasileiou, V Villasenor, L Weisgarberi, T Westerhoff, S Williams, DA Wisher, IG Wood, J Yodh, GB Younk, PW Zaborov, D Zepeda, A Zhou, H AF Abdo, A. A. Abeysekara, A. U. Alfaro, R. Allen, B. T. Alvarez, C. Alvarez, J. D. Arceo, R. Arteaga-Velazquez, J. C. Aune, T. Solares, H. A. Ayala Barber, A. S. Baughman, B. M. Bautista-Elivar, N. Gonzalez, J. Becerra Belmont, E. BenZvi, S. Y. Berley, D. Rosales, M. Bonilla Braun, J. Caballero-Lopez, R. A. Caballero-Mora, K. S. Carraminiana, A. Castillo, M. Christopher, G. E. Cotti, U. Cotzomi, J. De la Fuente, E. De Leon, C. DeYoung, T. Hernandez, R. Diaz Diaz-Cruz, K. L. Diaz-Velezi, J. C. Dingus, B. L. DuVernoisi, M. A. Ellsworth, R. W. Fiorinoi, D. W. Fraija, N. Galindo, A. Garfias, F. Gonzalez, M. M. Goodman, J. A. Grabski, V. Gussert, M. Hampel-Arias, Z. Harding, J. P. Hays, E. Hoffman, C. M. Hui, C. M. Huintemeyer, P. Imrani, A. Iriarte, A. Kam, P. Kieda, D. Kolterman, B. E. Kunde, Gj. Lara, A. Lauer, Rj. Lee, W. H. Lennarz, D. Vargas, H. Leon Linares, E. C. Linnemann, J. T. Longo, M. Luna-Garcla, R. MacGibbon, J. H. Marinelli, A. Marinelli, S. S. Martinez, H. Martinez, . Martinez-Castro, J. Matthews, J. A. J. McEnery, J. Torres, E. Mendoza Mincer, A. I. Miranda-Romagnoli, P. Moreno, E. Morgan, T. Mostafa, M. Nellen, L. Nemethy, P. Newbold, M. Noriega-Papaqui, R. Oceguera-Becerra, T. Patricelli, B. Pelayo, R. Perez-Perez, E. G. Pretz, J. Riviere, C. Rosa-Gonzalez, D. Ruiz-Velasco, E. Ryan, J. Salazar, H. Salesa, F. Sandoval, A. Parkinson, P. M. Saz Schneider, M. Silich, S. Sinnis, G. Smith, A. J. Stump, D. Woodle, K. Sparks Springer, R. W. Taboada, I. Toale, P. A. Tollefson, K. Torres, I. Ukwatta, T. N. Vasileiou, V. Villasenor, L. Weisgarberi, T. Westerhoff, S. Williams, D. A. Wisher, I. G. Wood, J. Yodh, G. B. Younk, P. W. Zaborov, D. Zepeda, A. Zhou, H. TI Milagro limits and HAWC sensitivity for the rate-density of evaporating Primordial Black Holes SO ASTROPARTICLE PHYSICS LA English DT Article DE Primordial Black Holes; HAWC; Milagro; Very High Energy Bursts ID GLUON-JET EMISSION; GAMMA-RAY BURSTS; COSMIC-RAYS; QUARK-JET AB Primordial Black Holes (PBHs) are gravitationally collapsed objects that may have been created by density fluctuations in the early universe and could have arbitrarily small masses down to the Planck scale. Hawking showed that due to quantum effects, a black hole has a temperature inversely proportional to its mass and will emit all species of fundamental particles thermally. PBHs with initial masses of similar to 5.0 x 10(14) g should be expiring in the present epoch with bursts of high-energy particles, including gamma radiation in the GeV-TeV energy range. The Milagro high energy observatory, which operated from 2000 to 2008, is sensitive to the high end of the PBH evaporation gamma-ray spectrum. Due to its large field-of-view, more than 90% duty cycle and sensitivity up to 100 TeV gamma rays, the Milagro observatory is well suited to perform a search for PBH bursts. Based on a search on the Milagro data, we report new PBH burst rate density upper limits over a range of PBH observation times. In addition, we report the sensitivity of the Milagro successor, the High Altitude Water Cherenkov (HAWC) observatory, to PBH evaporation events. Published by Elsevier B.V. C1 [Abdo, A. A.; Abeysekara, A. U.; DeYoung, T.; Linnemann, J. T.; Marinelli, S. S.; Stump, D.; Tollefson, K.; Ukwatta, T. N.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alfaro, R.; Grabski, V.; Vargas, H. Leon; Marinelli, A.; Oceguera-Becerra, T.; Ruiz-Velasco, E.; Sandoval, A.] Univ Nacl Autonoma Mexico, Inst Fis, Mexico City 01000, DF, Mexico. [Alvarez, C.; Arceo, R.] Univ Autonoma Chiapas, CEFyMAP, Chiapas, Mexico. [Alvarez, J. D.; Arteaga-Velazquez, J. C.; Cotti, U.; De Leon, C.; Linares, E. C.; Villasenor, L.] Univ Michoacana San Nicoltis Hidalgo, Morelia, Michoacan, Mexico. [Solares, H. A. Ayala; Hui, C. M.; Huintemeyer, P.; Zhou, H.] Michigan Technol Univ, Dept Phys, Houghton, MI 49931 USA. [Barber, A. S.; Kieda, D.; Newbold, M.; Springer, R. W.] Univ Utah, Dept Phys & Astron, Salt Lake City, UT USA. [Baughman, B. M.; Gonzalez, J. Becerra; Belmont, E.; Berley, D.; Braun, J.; Ellsworth, R. W.; Goodman, J. A.; Riviere, C.; Smith, A. J.; Vasileiou, V.; Wood, J.] Univ Maryland, Dept Phys, College Pk, MD 20742 USA. [Bautista-Elivar, N.; Perez-Perez, E. G.] Univ Politecn Pachuca, Pachuca, Hgo, Mexico. [Gonzalez, J. Becerra; Hays, E.; Lara, A.; McEnery, J.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Diaz-Velezi, J. C.; DuVernoisi, M. A.; Fiorinoi, D. W.; Hampel-Arias, Z.; Imrani, A.; Kam, P.; Weisgarberi, T.; Westerhoff, S.; Wisher, I. G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Rosales, M. Bonilla; Carraminiana, A.; Hernandez, R. Diaz; Galindo, A.; Torres, E. Mendoza; Rosa-Gonzalez, D.; Silich, S.; Torres, I.] Inst Nacl Astres Opt & Elect, Puebla, Mexico. [Caballero-Lopez, R. A.] Univ Nacl Autonoma Mexico, Inst Geofis, Mexico City 04510, DF, Mexico. [Caballero-Mora, K. S.; Martinez, H.; Zepeda, A.] IPN, Ctr Invest & Estudios Avanzados, Dept Phys, Mexico City 07738, DF, Mexico. [Castillo, M.; Cotzomi, J.; Diaz-Cruz, K. L.; Martinez, .; Moreno, E.; Salazar, H.] Benemerita Univ Autonoma Puebla, Fac Ciencias Fis Matemat, Puebla, Mexico. [De la Fuente, E.; Oceguera-Becerra, T.] Univ Guadalajara, IAMDpto Fis,Dpto Elect CUCEI,ITPhd CUCEA,Phys Mat, Guadalajara, Jalisco, Mexico. [DeYoung, T.; Mostafa, M.; Pretz, J.; Salesa, F.; Woodle, K. Sparks; Zaborov, D.] Penn State Univ, Dept Phys, University Pk, PA 16802 USA. [Dingus, B. L.; Harding, J. P.; Hoffman, C. M.; Kunde, Gj.; Sinnis, G.; Ukwatta, T. N.; Younk, P. W.] Los Alamos Natl Lab, Div Phys, Los Alamos, NM 87545 USA. [Ellsworth, R. W.] George Mason Univ, Sch Phys Astron & Computat Sci, Fairfax, VA 22030 USA. [Fraija, N.; Garfias, F.; Gonzalez, M. M.; Iriarte, A.; Lee, W. H.; Patricelli, B.; Riviere, C.] Univ Nacl Autonoma Mexico, Inst Astron, Mexico City 04510, DF, Mexico. [Gussert, M.; Longo, M.] Colorado State Univ, Dept Phys, Ft Collins, CO 80523 USA. [Lauer, Rj.; Matthews, J. A. J.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Lennarz, D.; Taboada, I.] Ctr Relativist Astrophys, Georgia Inst Technol, Atlanta, GA 30332 USA. [Lennarz, D.; Taboada, I.] Georgia Inst Technol, Sch Phys, Atlanta, GA 30332 USA. [Luna-Garcla, R.; Martinez-Castro, J.; Pelayo, R.] Ctr Invest Computac, Inst Politecn Nacl, Mexico City, DF, Mexico. [Miranda-Romagnoli, P.; Noriega-Papaqui, R.] Univ Autonoma Estado Hidalgo, Pachuca, Hgo, Mexico. [Nellen, L.] Univ Nacl Autenoma Mexico, Inst Ciencias Nucleares, Mexico City, DF, Mexico. [Ryan, J.] Univ New Hampshire, Ctr Space Sci, Durham, NH 03824 USA. [Aune, T.; Parkinson, P. M. Saz; Schneider, M.; Williams, D. A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Toale, P. A.] Univ Alabama, Dept Phys & Astron, Tuscaloosa, AL 35487 USA. [Allen, B. T.; Yodh, G. B.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. [MacGibbon, J. H.] Univ N Florida, Dept Phys, Jacksonville, FL 32224 USA. [BenZvi, S. Y.] Univ Rochester, Dept Phys & Astron, Rochester, NY 14627 USA. [Christopher, G. E.; Kolterman, B. E.; Mincer, A. I.; Nemethy, P.] New York Univ, Dept Phys, New York, NY 10003 USA. [Morgan, T.] Univ New Hampshire, Dept Phys, Durham, NH 03824 USA. [Parkinson, P. M. Saz] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. RP Ukwatta, TN (reprint author), Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. EM tilan.ukwatta@gmail.com OI Lara, Alejandro/0000-0001-6336-5291; Dingus, Brenda/0000-0001-8451-7450; Mincer, Allen/0000-0002-6307-1418; Becerra Gonzalez, Josefa/0000-0002-6729-9022 FU National Science Foundation; US Department of Energy Office of High-Energy Physics; LDRD program of Los Alamos National Laboratory; Consejo Nacional de Ciencia y Tecnologia [55155, 103520, 105033, 105666, 122331, 132197]; Red de Fisica de Altas Energias; DGAPA-UNAM [IG100414-3, IN108713, IN121309, IN115409]; VIEP-BUAP [161-EXC-2011]; University of Wisconsin Alumni Research Foundation; Luc Binette Foundation UNAM Postdoctoral Fellowship program; Institute of Geophysics and Planetary Physics at Los Alamos National Lab FX We gratefully acknowledge Scott De Lay his dedicated efforts in the construction and maintenance of the HAWC experiment. This work has been supported by: the National Science Foundation, the US Department of Energy Office of High-Energy Physics, the LDRD program of Los Alamos National Laboratory, Consejo Nacional de Ciencia y Tecnologia (Grants 55155, 103520, 105033, 105666, 122331 and 132197), Red de Fisica de Altas Energias, DGAPA-UNAM (Grants IG100414-3, IN108713 and IN121309, IN115409), VIEP-BUAP (Grant 161-EXC-2011), the University of Wisconsin Alumni Research Foundation, the Luc Binette Foundation UNAM Postdoctoral Fellowship program and the Institute of Geophysics and Planetary Physics at Los Alamos National Lab. Many of us are grateful for inspiring discussions with the late Donald Coyne on the subject of Primordial Black Holes. Finally, we thank the anonymous referee for comments that significantly improved the paper. NR 28 TC 7 Z9 7 U1 3 U2 21 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0927-6505 EI 1873-2852 J9 ASTROPART PHYS JI Astropart Phys. PD APR PY 2015 VL 64 BP 4 EP 12 DI 10.1016/j.astropartphys.2014.10.007 PG 9 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CA0SI UT WOS:000348626400002 ER PT J AU Gaisser, TK Klein, SR AF Gaisser, Thomas K. Klein, Spencer R. TI A new contribution to the conventional atmospheric neutrino flux SO ASTROPARTICLE PHYSICS LA English DT Article DE Atmospheric neutrinos; Neutrino astronomy; Neutral kaons ID SPECTRA; MUON AB Atmospheric neutrinos are an important background to astrophysical neutrino searches, and are also of considerable interest in their own right. This paper points out that the contribution to conventional atmospheric v(e) of the rare semileptonic decay of K-S becomes significant at high energy. Although the K-S -> pi ev branching ratio is very small, the short K-S lifetime leads to a high critical energy, so that, for vertical showers, the inclusion of K-S semileptonic decay increases the conventional v(e) flux by approximate to 30% at energies above 100 TeV. In this paper, we present calculations of the flux of v(e) from K-S. At energies above their critical energies, the v(e) fluxes from kaon decay may be simply related to the kaon semileptonic widths; this leads to a near-equality between the flux of v(e) from K+,K-L and K-S. (C) 2014 Elsevier B.V. All rights reserved. C1 [Gaisser, Thomas K.] Univ Delaware, Banal Res Inst, Newark, DE USA. [Gaisser, Thomas K.] Univ Delaware, Dept Phys & Astron, Newark, DE 19716 USA. [Klein, Spencer R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Klein, Spencer R.] Univ Calif Berkeley, Berkeley, CA 94720 USA. RP Klein, SR (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM gaisser@bartol.udel.edu; srklein@lbl.gov FU U.S. National Science Foundation [PHY-1307472, PHY-1205809]; U.S. Department of Energy [DE-AC-76SF00098, DE-FG02-12ER41808] FX We are grateful to David Seckel for calling our attention to the importance of kaon oscillations and regeneration in the context of this paper. and for his suggestions for the text. Work on this paper began while one of us (TKG) was participating in a program of the Munich Institute for Astro- and Particle Physics (MIAPP) of the DFG cluster of excellence "Origin and Structure of the Universe". This work was supported in part by U.S. National Science Foundation under Grants PHY-1307472 and PHY-1205809 and the U.S. Department of Energy under contract numbers DE-AC-76SF00098 and DE-FG02-12ER41808. NR 25 TC 4 Z9 4 U1 0 U2 3 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0927-6505 EI 1873-2852 J9 ASTROPART PHYS JI Astropart Phys. PD APR PY 2015 VL 64 BP 13 EP 17 DI 10.1016/j.astropartphys.2014.10.006 PG 5 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CA0SI UT WOS:000348626400003 ER PT J AU Guiseppe, VE Elliott, SR Fields, NE Hixon, D AF Guiseppe, V. E. Elliott, S. R. Fields, N. E. Hixon, D. TI Fast-neutron activation of long-lived nuclides in natural Pb SO ASTROPARTICLE PHYSICS LA English DT Article DE Neutron activation; Double-beta decay; Lead; Cosmic ray ID DOUBLE-BETA DECAY; GERMANIUM; FLUX AB We measured the production of the long-lived nuclides Bi-207, (202)pb, and Hg-194 in a sample of natural Pb due to high-energy neutron interactions using a neutron beam at the Los Alamos Neutron Science Center. The activated sample was counted by a HPGe detector to measure the amount of radioactive nuclides present. These nuclides are critical in understanding potential backgrounds in low background experiments utilizing large amounts of Pb shielding due to cosmogenic neutron interactions in the Pb while residing on the Earth's surface. By scaling the LANSCE neutron flux to a cosmic neutron flux, we measure the sea level cosmic ray production rates of 8.0 +/- 1.3 atoms/kg/day of Hg-194, 120 +/- 25 atoms/kg/day Pb-202, and <0.17 +/- 0.04 atoms/kg/day Bi-207. (C) 2014 Elsevier B.V. All rights reserved. C1 [Guiseppe, V. E.; Hixon, D.] Univ S Dakota, Vermillion, SD 57069 USA. [Elliott, S. R.; Fields, N. E.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Fields, N. E.] Univ Chicago, Chicago, IL 60637 USA. RP Guiseppe, VE (reprint author), Univ S Carolina, Columbia, SC 29208 USA. EM guiseppe@sc.edu FU U.S. Department of Energy, Office of Science, Office of Nuclear Physics [DE-SCOO05054]; LANL LDRD Program; DOE/NNSA Stewardship Science Graduate Fellowship Program [DE-FC52-08NA28752]; U.S. Department of Energy [DE-AC52-06NA25396]; Nuclear Physics office of the U.S. Department of Energy [2011LANLE9BW] FX This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics under Award Number DE-SCOO05054, the LANL LDRD Program, and the DOE/NNSA Stewardship Science Graduate Fellowship Program under Grant No. DE-FC52-08NA28752. This work benefited from the use of the Los Alamos Neutron Science Center, funded by the U.S. Department of Energy under contract DE-AC52-06NA25396. This work also benefited from our underground laboratory at the Waste Isolation Pilot Plant (WIPP), which we operate with support from the Nuclear Physics office of the U.S. Department of Energy under contract number 2011LANLE9BW. Finally, we thank our friends and hosts at the Waste Isolation Pilot Plant (WIPP) for their continuing support of our activities underground at that facility. NR 23 TC 1 Z9 1 U1 0 U2 3 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0927-6505 EI 1873-2852 J9 ASTROPART PHYS JI Astropart Phys. PD APR PY 2015 VL 64 BP 34 EP 39 DI 10.1016/j.astropartphys.2014.11.002 PG 6 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CA0SI UT WOS:000348626400005 ER PT J AU Yang, Y Li, XS Yang, F Zhang, W Zhang, X Ren, Y AF Yang, Ying Li, Xinsong Yang, Feng Zhang, Wen Zhang, Xin Ren, Yang TI New route toward integrating large nickel nanocrystals onto mesoporous carbons SO APPLIED CATALYSIS B-ENVIRONMENTAL LA English DT Article DE Nickel nanocrystals; Mesoporous carbon; Soft-templating approach; 4-Nitrophenol reduction; Magnetic separation ID HIGH CATALYTIC-ACTIVITY; RAY-ABSORPTION SPECTROSCOPY; ONE-POT SYNTHESIS; 4-NITROPHENOL REDUCTION; P-NITROPHENOL; NANOPARTICLES; SILICA; HYDROGENATION; FABRICATION; CONVERSION AB Integrating large and magnetic transition metal nanocrystals onto mesoporous carbons is of great importance owing to their low cost, easy separation and great potential in various applications. Herein we firstly report large nickel nanocrystals (Ni NCs, 30-75 nm) in situ integrated onto mesoporous carbons (MC), synthesized via block copolymer-directed self-assembly of nickel acetate and 8-quinolinol modified chitosan under neutral conditions assisted by tetraethyl orthosilicate before pyrolysis and silica removal. This neutral one-pot synthesis not only renders evenly dispersed Ni NCs firmly attached on the mesoporous carbonaceous framework without using any stabilizer, but also creates larger Ni NCs as compared to those prepared by acidic and basic synthetic routes. It is found that all nickel catalysts can be magnetically separated easily; and the Ni NC size, microstructure and the carbonaceous support morphology are well adjusted by variation of the pyrolysis temperature, which in turn affects the catalytic properties of Ni NCs towards 4-nitrophenol reduction. The Ni NC functionalized mesoporous carbon pyrolyzed at 750 degrees C (Ni-MC-750) simultaneously possessing twinned microstructure and carbon nanotube morphology, exhibits the highest catalytic efficiency. High-energy X-ray diffraction, N-2 adsorption/desorption, transmission electron microscopy, infrared spectroscopy, X-ray absorption fine structure and Raman spectroscopy studies, as well as the comparative catalytic tests have demonstrated these points. (C) 2014 Elsevier B.V. All rights reserved. C1 [Yang, Ying; Li, Xinsong; Yang, Feng; Zhang, Wen; Zhang, Xin] China Univ Petr, State Key Lab Heavy Oil Proc, Beijing 102249, Peoples R China. [Ren, Yang] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. RP Yang, Y (reprint author), China Univ Petr, State Key Lab Heavy Oil Proc, 18 Fuxue Rd, Beijing 102249, Peoples R China. EM catalyticscience@163.com; zhangxin@cup.edu.cn FU National Natural Science Foundation of China [21303229, 21173269, 91127040, 51101170]; Science Foundation of China University of Petroleum, Beijing [2462013YJRC018]; US Department of Energy-Basic Energy Sciences; NSERC; University of Washington; Canadian Light Source and the Advanced Photon Source; U.S. DOE [DE-AC02-06CH11357] FX Financial support for this research work from the National Natural Science Foundation of China (21303229, 21173269, 91127040 and 51101170), and the Science Foundation of China University of Petroleum, Beijing (2462013YJRC018) is acknowledged. PNC/XSD facilities at the Advanced Photon Source, and research at these facilities, are supported by the US Department of Energy-Basic Energy Sciences, a Major Resources Support grant from NSERC, the University of Washington, the Canadian Light Source and the Advanced Photon Source. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. We thank Dr. C.J. Sun for his kind support on EXAFS measurements at Sector 20. NR 63 TC 3 Z9 3 U1 4 U2 88 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0926-3373 EI 1873-3883 J9 APPL CATAL B-ENVIRON JI Appl. Catal. B-Environ. PD APR PY 2015 VL 165 BP 94 EP 102 DI 10.1016/j.apcatb.2014.09.056 PG 9 WC Chemistry, Physical; Engineering, Environmental; Engineering, Chemical SC Chemistry; Engineering GA AY4ZU UT WOS:000347584200012 ER PT J AU Zhao, NZ Zhou, YY Samson, EL AF Zhao, Naizhuo Zhou, Yuyu Samson, Eric L. TI Correcting Incompatible DN Values and Geometric Errors in Nighttime Lights Time-Series Images SO IEEE TRANSACTIONS ON GEOSCIENCE AND REMOTE SENSING LA English DT Article DE Geometric error; gross domestic product (GDP); nighttime lights development/decay; nighttime lights time-series (NLT) images ID SATELLITE IMAGERY; URBANIZATION DYNAMICS; POPULATION-DENSITY; URBAN DECLINE; UNITED-STATES; CITIES; CHINA; CONSUMPTION; CENSUS AB The Defense Meteorological Satellite Program's Operational Linescan System (DMSP-OLS) nighttime lights imagery has proven to be a powerful remote sensing tool to monitor urbanization and assess socioeconomic activities at large scales. However, the existence of incompatible digital number (DN) values and geometric errors severely limit application of nighttime light image data on multiyear quantitative research. In this paper, we extend and improve previous studies on intercalibrating nighttime lights image data to obtain more compatible and reliable nighttime lights time-series (NLT) image data for China and the U.S. through four steps, namely, intercalibration, geometric correction, steady-increase adjustment, and population data correction. We then use gross domestic product (GDP) data to test the processed NLT image data indirectly and find that sum light (summed DN value of pixels in a nighttime light image) maintains apparent increase trends with relatively large GDP growth rates but does not increase or decrease with relatively small GDP growth rates. As nighttime light is a sensitive indicator for economic activity, the temporally consistent trends between sum light and GDP growth rate imply that brightness of nighttime lights on the ground is correctly represented by the processed NLT image data. Finally, through analyzing the corrected NLT image data from 1992 to 2008, we find that China experienced apparent nighttime lights development in 1992-1997 and 2001-2008, respectively, and the U.S. showed nighttime lights decay in large areas after 2001. C1 [Zhao, Naizhuo] Texas Tech Univ, Dept Geosci, Lubbock, TX 79409 USA. [Zhou, Yuyu] Pacific NW Natl Lab, Global Change Res Inst, College Pk, MD 20749 USA. [Samson, Eric L.] Mayan Esteem Project, Farmington, CT 06032 USA. RP Zhou, YY (reprint author), Pacific NW Natl Lab, Global Change Res Inst, College Pk, MD 20749 USA. EM yuyu.zhou@pnnl.gov FU NASA ROSES Land-Cover/Land-Use Change Program [NNH11ZDA001N-LCLUC] FX This work was supported by the NASA ROSES Land-Cover/Land-Use Change Program under Grant NNH11ZDA001N-LCLUC. (Corresponding author: Yuyu Zhou.) NR 40 TC 7 Z9 7 U1 6 U2 63 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0196-2892 EI 1558-0644 J9 IEEE T GEOSCI REMOTE JI IEEE Trans. Geosci. Remote Sensing PD APR PY 2015 VL 53 IS 4 BP 2039 EP 2049 DI 10.1109/TGRS.2014.2352598 PG 11 WC Geochemistry & Geophysics; Engineering, Electrical & Electronic; Remote Sensing; Imaging Science & Photographic Technology SC Geochemistry & Geophysics; Engineering; Remote Sensing; Imaging Science & Photographic Technology GA AR9NQ UT WOS:000343902300030 ER PT J AU Moore, T Finley, P Brodsky, N Brown, T Apelberg, B Ambrose, B Glass, R AF Moore, Thomas Finley, Patrick Brodsky, Nancy Brown, Theresa Apelberg, Benjamin Ambrose, Bridget Glass, Robert TI Modeling Education and Advertising with Opinion Dynamics SO JASSS-THE JOURNAL OF ARTIFICIAL SOCIETIES AND SOCIAL SIMULATION LA English DT Article DE Opinion Dynamics; Social Networks; Media; Advertising ID ADOLESCENT SMOKING; MOVIES AB We present a modified Deffuant-Weisbuch opinion dynamics model that integrates the influence of media campaigns on opinion. Media campaigns promote messages intended to inform and influence the opinions of the targeted audiences through factual and emotional appeals. Media campaigns take many forms: brand-specific advertisements, promotions, and sponsorships, political, religious, or social messages, and public health and educational communications. We illustrate model-based analysis of campaigns using tobacco advertising and public health education as examples. In this example, "opinion" is not just an individual's attitude towards smoking, but the integration of a wide range of factors that influence the likelihood that an individual will decide to smoke, such as knowledge, perceived risk, perceived utility and affective evaluations of smoking. This model captures the ability of a media campaign to cause a shift in network-level average opinion, and the inability of a media message to do so if it promotes too extreme a viewpoint for a given target audience. Multiple runs displayed strong heterogeneity in response to media campaigns as the difference between network average initial opinion and broadcasted media opinion increased, with some networks responding ideally and others being largely unaffected. In addition, we show that networks that display community structure can be made more susceptible to be influenced by a media campaign by a complementary campaign focused on increasing tolerance to other opinions in targeted nodes with high betweenness centrality. Similarly, networks can be "inoculated" against advertising campaigns by a media campaign that decreases tolerance. C1 [Moore, Thomas; Finley, Patrick; Brodsky, Nancy; Brown, Theresa; Glass, Robert] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Apelberg, Benjamin; Ambrose, Bridget] US FDA, Ctr Tobacco Prod, Rockville, MD 20850 USA. RP Moore, T (reprint author), Sandia Natl Labs, POB 5800,MS 1138, Albuquerque, NM 87185 USA. EM tmoore@sandia.gov; pdfinle@sandia.gov; nsbrods@sandia.gov; tjbrown@sandia.gov; benjamin.apelberg@fda.hhs.gov; bridget.ambrose@fda.hhs.gov; rjglass@sandia.gov FU U.S. Food and Drug Administration; U.S. Department of Energy/Sandia National Laboratories [224109011]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was funded by the U.S. Food and Drug Administration through a contract with the U.S. Department of Energy/Sandia National Laboratories (funding document 224109011). Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. The funders, other than employees named as authors or described in the acknowledgments, had no role in the study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 39 TC 0 Z9 0 U1 0 U2 3 PU J A S S S PI GUILDFORD PA UNIV SURREY, DEPT SOCIOLOGY, GUILDFORD GU2 7XH, SURREY, ENGLAND SN 1460-7425 J9 JASSS-J ARTIF SOC S JI JASSS PD MAR 31 PY 2015 VL 18 IS 2 AR 7 PG 11 WC Social Sciences, Interdisciplinary SC Social Sciences - Other Topics GA CH9RL UT WOS:000354373800011 ER PT J AU Gilbert, JA AF Gilbert, Jack A. TI Social behavior and the microbiome SO ELIFE LA English DT Editorial Material ID ENVIRONMENT C1 [Gilbert, Jack A.] Argonne Natl Lab, Dept Biosci, Chicago, IL 60439 USA. [Gilbert, Jack A.] Argonne Natl Lab, Inst Genom & Syst Biol, Chicago, IL USA. [Gilbert, Jack A.] Univ Chicago, Dept Ecol & Evolut, Chicago, IL 60637 USA. [Gilbert, Jack A.] Univ Chicago, Dept Surg, Chicago, IL 60637 USA. RP Gilbert, JA (reprint author), Argonne Natl Lab, Dept Biosci, Chicago, IL 60439 USA. EM gilbertjack@anl.gov NR 7 TC 0 Z9 0 U1 10 U2 24 PU ELIFE SCIENCES PUBLICATIONS LTD PI CAMBRIDGE PA SHERATON HOUSE, CASTLE PARK, CAMBRIDGE, CB3 0AX, ENGLAND SN 2050-084X J9 ELIFE JI eLife PD MAR 31 PY 2015 VL 4 AR e07322 DI 10.7554/eLife.07322 PG 3 WC Biology SC Life Sciences & Biomedicine - Other Topics GA CE7LP UT WOS:000352022100006 ER PT J AU Nagarkar-Jaiswal, S Lee, PT Campbell, ME Chen, KC Anguiano-Zarate, S Gutierrez, MC Busby, T Lin, WW He, YC Schulze, KL Booth, BW Evans-Holm, M Venken, KJT Levis, RW Spradling, AC Hoskins, RA Bellen, HJ AF Nagarkar-Jaiswal, Sonal Lee, Pei-Tseng Campbell, Megan E. Chen, Kuchuan Anguiano-Zarate, Stephanie Gutierrez, Manuel Cantu Busby, Theodore Lin, Wen-Wen He, Yuchun Schulze, Karen L. Booth, Benjamin W. Evans-Holm, Martha Venken, Koen J. T. Levis, Robert W. Spradling, Allan C. Hoskins, Roger A. Bellen, Hugo J. TI A library of MiMICs allows tagging of genes and reversible, spatial and temporal knockdown of proteins in Drosophila SO ELIFE LA English DT Article ID NEUROMUSCULAR-JUNCTION; ALPHA-CATENIN; ACTIVE ZONES; MELANOGASTER; MEMORY; RESOURCE; SYSTEM; GENOME; DUNCE; TOOL AB Here, we document a collection of similar to 7434 MiMIC (Minos Mediated Integration Cassette) insertions of which 2854 are inserted in coding introns. They allowed us to create a library of 400 GFP-tagged genes. We show that 72% of internally tagged proteins are functional, and that more than 90% can be imaged in unfixed tissues. Moreover, the tagged mRNAs can be knocked down by RNAi against GFP (iGFPi), and the tagged proteins can be efficiently knocked down by deGradFP technology. The phenotypes associated with RNA and protein knockdown typically correspond to severe loss of function or null mutant phenotypes. Finally, we demonstrate reversible, spatial, and temporal knockdown of tagged proteins in larvae and adult flies. This new strategy and collection of strains allows unprecedented in vivo manipulations in flies for many genes. These strategies will likely extend to vertebrates. C1 [Nagarkar-Jaiswal, Sonal; Lee, Pei-Tseng; Campbell, Megan E.; Anguiano-Zarate, Stephanie; Gutierrez, Manuel Cantu; Busby, Theodore; Lin, Wen-Wen; Bellen, Hugo J.] Baylor Coll Med, Dept Mol & Human Genet, Houston, TX 77030 USA. [Chen, Kuchuan; Bellen, Hugo J.] Baylor Coll Med, Program Dev Biol, Houston, TX 77030 USA. [He, Yuchun; Schulze, Karen L.; Bellen, Hugo J.] Baylor Coll Med, Howard Hughes Med Inst, Houston, TX 77030 USA. [Booth, Benjamin W.; Evans-Holm, Martha; Hoskins, Roger A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. [Venken, Koen J. T.] Baylor Coll Med, Verna & Marrs McLean Dept Biochem & Mol Biol, Houston, TX 77030 USA. [Levis, Robert W.; Spradling, Allan C.] Carnegie Inst Sci, Dept Embryol, Howard Hughes Med Inst, Baltimore, MD 21210 USA. [Bellen, Hugo J.] Texas Childrens Hosp, Jan & Dan Duncan Neurol Res Inst, Houston, TX 77030 USA. [Bellen, Hugo J.] Baylor Coll Med, Dept Neurosci, Houston, TX 77030 USA. RP Bellen, HJ (reprint author), Baylor Coll Med, Dept Mol & Human Genet, Houston, TX 77030 USA. EM hbellen@bcm.edu RI Venken, Koen/B-9909-2013 OI Venken, Koen/0000-0003-0741-4698 FU National Institute of General Medical Sciences (NIGMS); National Institute of Child Health and Human Development (NICHD) [R01GM067858]; March of Dimes Foundation [3R01GM067858-11S1, 1-FY14-315]; Cancer Prevention and Research Institute of Texas (CPRIT); National Human Genome Research Institute (NHGRI); National Institute of General Medical Sciences (NIGMS) [3R01GM067858-09S1]; Baylor College of Medicine; National Institutes of Health (NIH) [1R21GM110190] FX National Institute of General Medical Sciences (NIGMS) Sonal Nagarkar-Jaiswal, Pei-Tseng Lee, Megan E Campbell, Stephanie Anguiano-Zarate, Manuel Cantu Gutierrez, Theodore Busby, Wen-Wen Lin, Benjamin W Booth, Martha Evans-Holm, Robert W Levis, Allan C Spradling, Roger A Hoskins, Hugo J Bellen; National Institute of Child Health and Human Development (NICHD) R01GM067858 Hugo J Bellen; March of Dimes Foundation 3R01GM067858-11S1 Stephanie Anguiano-Zarate; Cancer Prevention and Research Institute of Texas (CPRIT) Koen JT Venken; National Human Genome Research Institute (NHGRI) Koen JT Venken, Roger A Hoskins; National Institute of General Medical Sciences (NIGMS) 3R01GM067858-09S1 Theodore Busby; Baylor College of Medicine McNair Startup Funds Koen JT Venken; March of Dimes Foundation #1-FY14-315 Koen JT Venken; National Institutes of Health (NIH) 1R21GM110190 Koen JT Venken NR 65 TC 34 Z9 34 U1 0 U2 14 PU ELIFE SCIENCES PUBLICATIONS LTD PI CAMBRIDGE PA SHERATON HOUSE, CASTLE PARK, CAMBRIDGE, CB3 0AX, ENGLAND SN 2050-084X J9 ELIFE JI eLife PD MAR 31 PY 2015 VL 4 AR e05338 DI 10.7554/eLife.05338 PG 28 WC Biology SC Life Sciences & Biomedicine - Other Topics GA CE7LP UT WOS:000352022100001 ER PT J AU Troparevsky, MC Morris, JR Kent, PRC Lupini, AR Stocks, GM AF Troparevsky, M. Claudia Morris, James R. Kent, Paul R. C. Lupini, Andrew R. Stocks, G. Malcolm TI Criteria for Predicting the Formation of Single-Phase High-Entropy Alloys SO PHYSICAL REVIEW X LA English DT Article ID SOLID-SOLUTION; AMORPHOUS PHASE; MICROSTRUCTURE; STABILITY; IRON; BEHAVIOR; DESIGN AB High-entropy alloys constitute a new class of materials whose very existence poses fundamental questions regarding the physical principles underlying their unusual phase stability. Originally thought to be stabilized by the large entropy of mixing associated with their large number of components (five or more), these alloys have attracted attention for their potential applications. Yet, no model capable of robustly predicting which combinations of elements will form a single phase currently exists. Here, we propose a model that, through the use of high-throughput computation of the enthalpies of formation of binary compounds, predicts specific combinations of elements most likely to form single-phase, high-entropy alloys. The model correctly identifies all known single-phase alloys while rejecting similar elemental combinations that are known to form an alloy comprising multiple phases. In addition, we predict numerous potential single-phase alloy compositions and provide three tables with the ten most likely five-, six-, and seven-component single-phase alloys to guide experimental searches. C1 [Troparevsky, M. Claudia; Morris, James R.; Lupini, Andrew R.; Stocks, G. Malcolm] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Morris, James R.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Kent, Paul R. C.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Kent, Paul R. C.] Oak Ridge Natl Lab, Div Math & Comp Sci, Oak Ridge, TN 37831 USA. RP Troparevsky, MC (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RI Kent, Paul/A-6756-2008; Morris, J/I-4452-2012; Stocks, George Malcollm/Q-1251-2016 OI Kent, Paul/0000-0001-5539-4017; Morris, J/0000-0002-8464-9047; Stocks, George Malcollm/0000-0002-9013-260X FU U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division; ORNL's Center for Nanophase Materials Sciences (CNMS); Scientific User Facilities Division (PRCK), Basic Energy Sciences, U.S. Department of Energy; ORNL, BES FX Research was supported by the U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division (M.C.T., G.M.S., J.R.M., and A.R.L.) and through a user project supported by ORNL's Center for Nanophase Materials Sciences (CNMS), which is sponsored by the Scientific User Facilities Division (PRCK), Basic Energy Sciences, U.S. Department of Energy. Calculations were performed on ORNL, BES funded, clusters and at the National Energy Research Scientific Computing Center (NERSC). NR 41 TC 43 Z9 43 U1 31 U2 111 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2160-3308 J9 PHYS REV X JI Phys. Rev. X PD MAR 31 PY 2015 VL 5 IS 1 AR 011041 DI 10.1103/PhysRevX.5.011041 PG 6 WC Physics, Multidisciplinary SC Physics GA CE8AT UT WOS:000352063800002 ER PT J AU Mohagheghi, A Linger, JG Yang, SH Smith, H Dowe, N Zhang, M Pienkos, PT AF Mohagheghi, Ali Linger, Jeffrey G. Yang, Shihui Smith, Holly Dowe, Nancy Zhang, Min Pienkos, Philip T. TI Improving a recombinant Zymomonas mobilis strain 8b through continuous adaptation on dilute acid pretreated corn stover hydrolysate SO BIOTECHNOLOGY FOR BIOFUELS LA English DT Article DE Zymomonas mobilis; Xylose; Pretreated corn stover; Adaptation; Turbidostat; Next-generation sequencing (NGS) ID GROWTH; DEACETYLATION; TOLERANCE; ETHANOL AB Background: Complete conversion of the major sugars of biomass including both the C-5 and C-6 sugars is critical for biofuel production processes. Several inhibitory compounds like acetate, hydroxymethylfurfural (HMF), and furfural are produced from the biomass pretreatment process leading to 'hydrolysate toxicity,' a major problem for microorganisms to achieve complete sugar utilization. Therefore, development of more robust microorganisms to utilize the sugars released from biomass under toxic environment is critical. In this study, we use continuous culture methodologies to evolve and adapt the ethanologenic bacterium Zymomonas mobilis to improve its ethanol productivity using corn stover hydrolysate. Results: A turbidostat was used to adapt the Z. mobilis strain 8b in the pretreated corn stover liquor. The adaptation was initiated using pure sugar (glucose and xylose) followed by feeding neutralized liquor at different dilution rates. Once the turbidostat reached 60% liquor content, the cells began washing out and the adaptation was stopped. Several 'sub-strains' were isolated, and one of them, SS3 (sub-strain 3), had 59% higher xylose utilization than the parent strain 8b when evaluated on 55% neutralized PCS (pretreated corn stover) liquor. Using saccharified PCS slurry generated by enzymatic hydrolysis from 25% solids loading, SS3 generated an ethanol yield of 75.5% compared to 64% for parent strain 8b. Furthermore, the total xylose utilization was 57.7% for SS3 versus 27.4% for strain 8b. To determine the underlying genotypes in these new sub-strains, we conducted genomic resequencing and identified numerous single-nucleotide mutations (SNPs) that had arisen in SS3. We further performed quantitative reverse transcription PCR (qRT-PCR) on genes potentially affected by these SNPs and identified significant downregulation of two genes, ZMO0153 and ZMO0776, in SS3 suggesting potential genetic mechanisms behind SS3's improved performance. Conclusion: We have adapted/evolved Z. mobilis strain 8b for enhanced tolerance to the toxic compounds present in corn stover hydrolysates. The adapted strain SS3 has higher xylose utilization rate and produce more ethanol than the parent strain. We have identified transcriptional changes which may be responsible for these phenotypes, providing foundations for future research directions in improving Z. mobilis as biocatalysts for the production of ethanol or other fuel precursors. C1 [Mohagheghi, Ali; Linger, Jeffrey G.; Yang, Shihui; Smith, Holly; Dowe, Nancy; Zhang, Min; Pienkos, Philip T.] Natl Bioenergy Ctr, Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Mohagheghi, A (reprint author), Natl Bioenergy Ctr, Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. EM Ali.Mohagheghi@nrel.gov FU Bioenergy Technologies Office (BETO), a subdivision within the U.S. Department of Energy's (DOE's) Office of Energy Efficiency and Renewable Energy (EERE) FX We would like to acknowledge funding support from the Bioenergy Technologies Office (BETO), a subdivision within the U.S. Department of Energy's (DOE's) Office of Energy Efficiency and Renewable Energy (EERE). The authors also would like to thank NREL Biomass Analysis Team (BAT) for helping at different stage of the project on sample analysis. NR 25 TC 5 Z9 5 U1 6 U2 20 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1754-6834 J9 BIOTECHNOL BIOFUELS JI Biotechnol. Biofuels PD MAR 31 PY 2015 VL 8 AR 55 DI 10.1186/s13068-015-0233-z PG 9 WC Biotechnology & Applied Microbiology; Energy & Fuels SC Biotechnology & Applied Microbiology; Energy & Fuels GA CE7XS UT WOS:000352055800001 PM 25834640 ER PT J AU Qian, F Pascall, AJ Bora, M Han, TYJ Guo, SR Ly, SS Worsley, MA Kuntz, JD Olson, TY AF Qian, Fang Pascall, Andrew J. Bora, Mihail Han, T. Yong-Jin Guo, Shirui Ly, Sonny S. Worsley, Marcus A. Kuntz, Joshua D. Olson, Tammy Y. TI On-Demand and Location Selective Particle Assembly via Electrophoretic Deposition for Fabricating Structures with Particle-to-Particle Precision SO LANGMUIR LA English DT Article ID PATTERNED SURFACES; COLLOIDAL CRYSTALLIZATION; ELECTRON-MICROSCOPY; GOLD NANOPARTICLES; PHOTONIC CRYSTALS; SUPERLATTICES; ARRAYS; TEMPLATE; NANOTECHNOLOGY; COMPOSITES AB Programmable positioning of 2 pm polystyrene (PS) beads with single particle precision and location selective, "on-demand", particle deposition was demonstrated by utilizing patterned electrodes and electrophoretic deposition (EPD). An electrode with differently sized hole patterns, from 0.5 to 5 pm, was used to illustrate the discriminatory particle deposition events based on the voltage and particle-to-hole size ratio. With decreasing patterned hole size, a larger electric field was required for a particle deposition event to occur in that hole. For the 5 pm hole, particle deposition began to occur at 10 V/cm where as an electric field of 15 V/cm was required for particles to begin depositing in the 2 pm holes. The likelihood of particle depositions continued to increase for smaller sized holes as the electric field increased. Eventually, a monolayer of particles began to form at approximately 20 V/cm. In essence, a voltage threshold was found for each hole pattern of different sizes, allowing fine adjustments in pattern hole size and voltage to control when a particle deposition event took place, even with the patterns on the same electrode. This phenomenon opens a route toward controlled, multimaterial deposition and assembly onto substrates without repatterning of the electrode or complicated surface modification of the particles. An analytical approach using the theories for electrophoresis and dielectrophoresis found the former to be the dominating force for depositing a particle into a patterned hole. Ebeam lithography was used to pattern spherical holes in precise configurations onto electrode surfaces, where each hole accompanied a polystyrene (PS) particle placement and attachment during EPD. The versatility of e-beam lithography was utilized to create arbitrary pattern configurations to fabricate particle assemblies of limitless configurations, enabling fabrication of unique materials assemblies and interfaces. C1 [Qian, Fang; Pascall, Andrew J.; Bora, Mihail; Han, T. Yong-Jin; Guo, Shirui; Ly, Sonny S.; Worsley, Marcus A.; Kuntz, Joshua D.; Olson, Tammy Y.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RP Olson, TY (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94551 USA. EM olson43@llnl.gov OI Worsley, Marcus/0000-0002-8012-7727 FU US Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Laboratory Directed Research and Development Program at LLNL [13-LW-066, 14-SI-004] FX This work performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. The project was funded by the Laboratory Directed Research and Development Program at LLNL (13-LW-066, 14-SI-004). We thank Dr. Adam Schwartzberg of Lawrence Berkeley National Laboratory and Dr. Kyle T. Sullivan and Dr. Luis Zepeda-Ruiz of Lawrence Livermore National Laboratory for their helpful discussions. NR 60 TC 6 Z9 6 U1 9 U2 60 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0743-7463 J9 LANGMUIR JI Langmuir PD MAR 31 PY 2015 VL 31 IS 12 BP 3563 EP 3568 DI 10.1021/la502724n PG 6 WC Chemistry, Multidisciplinary; Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CF0OZ UT WOS:000352245400001 PM 25314133 ER PT J AU Delaire, O Al-Qasir, II May, AF Li, CW Sales, BC Niedziela, JL Ma, J Matsuda, M Abernathy, DL Berlijn, T AF Delaire, O. Al-Qasir, I. I. May, A. F. Li, C. W. Sales, B. C. Niedziela, J. L. Ma, J. Matsuda, M. Abernathy, D. L. Berlijn, T. TI Heavy-impurity resonance, hybridization, and phonon spectral functions SO PHYSICAL REVIEW B LA English DT Article ID TOTAL-ENERGY CALCULATIONS; FORCE-CONSTANT CHANGES; AUGMENTED-WAVE METHOD; ELECTRONIC-STRUCTURE; EPSILON-FESI; THERMOELECTRIC-MATERIALS; STATIC COMPRESSION; VIBRATIONAL-MODES; THERMAL DISORDER; IRON SILICIDE AB The vibrational behavior of heavy substitutional impurities (M = Ir, Os) in Fe1-xMxSi (x = 0,0.02,0.04,0.1) was investigated with a combination of inelastic neutron scattering (INS), transport measurements, and first-principles simulations. Our INS measurements on single crystals mapped the four-dimensional dynamical structure factor, S(Q, E), for several compositions and temperatures. Our results show that both Ir and Os impurities lead to the formation of a weakly dispersive resonance vibrational mode, in the energy range of the acoustic phonon dispersions of the FeSi host. We also show that Ir doping, which introduces free carriers, leads to softened interatomic force constants compared to doping with Os, which is isoelectronic to Fe. We analyze the phonon S(Q, E) from INS through a Green's-function model incorporating the phonon self-energy based on first-principles density functional theory simulations, and we study the disorder-induced lifetimes on large supercells. Calculations of the quasiparticle spectral functions in the doped system reveal the hybridization between the resonance and the acoustic phonon modes. Our results demonstrate a strong interaction of the host acoustic dispersions with the resonance mode, likely leading to the large observed suppression in lattice thermal conductivity. C1 [Delaire, O.; Al-Qasir, I. I.; May, A. F.; Li, C. W.; Sales, B. C.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Niedziela, J. L.] Oak Ridge Natl Lab, Instrument & Source Div, Oak Ridge, TN 37831 USA. [Ma, J.; Matsuda, M.; Abernathy, D. L.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Berlijn, T.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Berlijn, T.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. RP Delaire, O (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. EM delaireoa@ornl.gov RI Abernathy, Douglas/A-3038-2012; May, Andrew/E-5897-2011; Ma, Jie/C-1637-2013; Berlijn, Tom/A-3859-2016; Matsuda, Masaaki/A-6902-2016; BL18, ARCS/A-3000-2012 OI Abernathy, Douglas/0000-0002-3533-003X; May, Andrew/0000-0003-0777-8539; Berlijn, Tom/0000-0002-1001-2238; Matsuda, Masaaki/0000-0003-2209-9526; FU US Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division, through the Office of Science Early Career Research Program; US Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; US Department of Energy, Office of Basic Energy Sciences, S3TEC Energy Frontier Research Center, DOE [DE-SC0001299]; Laboratory Directed Research and Development Program of ORNL; Wigner Fellow at the Oak Ridge National Laboratory; US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division; Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy; Office of Science of the US Department of Energy [DE-AC02-05CH11231] FX Neutron-scattering work by O.D. was supported by the US Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division, through the Office of Science Early Career Research Program. A.F.M. and B.C.S. were supported by the US Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. J.M. and C.W.L. were supported by the US Department of Energy, Office of Basic Energy Sciences, as part of the S3TEC Energy Frontier Research Center, DOE Grant No. DE-SC0001299. I.I.A. was sponsored by the Laboratory Directed Research and Development Program of ORNL. T.B. was supported as a Wigner Fellow at the Oak Ridge National Laboratory. The phonon modeling work was performed within the Center for Accelerating Materials Modeling of SNS data, supported by the US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division (J.L.N., O.D.). The research at Oak Ridge National Laboratory's Spallation Neutron Source and High Flux Isotope Reactor was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. This research used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the US Department of Energy under Contract No. DE-AC02-05CH11231. NR 77 TC 8 Z9 8 U1 3 U2 36 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 31 PY 2015 VL 91 IS 9 AR 094307 DI 10.1103/PhysRevB.91.094307 PG 12 WC Physics, Condensed Matter SC Physics GA CE7ZE UT WOS:000352059700001 ER PT J AU Zhong, X Rungger, I Zapol, P Heinonen, O AF Zhong, X. Rungger, I. Zapol, P. Heinonen, O. TI Electronic and magnetic properties of Ti4O7 predicted by self-interaction-corrected density functional theory SO PHYSICAL REVIEW B LA English DT Article ID METAL-INSULATOR TRANSITIONS; CHARGE ORDER; PHOTOCATALYSIS; LOCALIZATION; PRINCIPLES; MEMORY; TI2O3 AB Understanding electronic properties of substoichiometric phases of titanium oxide such as Magneli phase Ti4O7 is crucial in designing and modeling resistive switching devices. Here we present our study on Magneli phase Ti4O7 together with rutile TiO2 and Ti2O3 using density functional theory methods with atomic-orbital-based self-interaction correction (ASIC). We predict a new antiferromagnetic (AF) ground state in the low temperature (LT) phase, and we explain energy difference with a competing AF state using a Heisenberg model. The predicted energy ordering of these states in the LT phase is calculated to be robust in a wide range of modeled isotropic strain. We have also investigated the dependence of the electronic structures of the Ti-O phases on stoichiometry. The splitting of titanium t(2g) orbitals is enhanced with increasing oxygen deficiency as Ti-O is reduced. The electronic properties of all these phases can be reasonably well described by applying ASIC with a "standard" value for transition metal oxides of the empirical parameter alpha of 0.5 representing the magnitude of the applied self-interaction correction. C1 [Zhong, X.; Zapol, P.; Heinonen, O.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Rungger, I.] Univ Dublin Trinity Coll, Sch Phys, AMBER, Dublin 2, Ireland. [Rungger, I.] Univ Dublin Trinity Coll, CRANN, Dublin 2, Ireland. [Heinonen, O.] Northwestern Univ, Ctr Hierarch Mat Design, Evanston, IL 60208 USA. RP Zhong, X (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. RI Zapol, Peter/G-1810-2012; Zhong, Xiaoliang/B-2220-2012; OI Zapol, Peter/0000-0003-0570-9169; Heinonen, Olle/0000-0002-3618-6092 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Materials Science and Engineering [DE-AC02-06CH11357]; EU [FP7-FET GA618082] FX Work at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Materials Science and Engineering under Contract No. DE-AC02-06CH11357. I.R. acknowledges financial support from the EU project ACMOL (FP7-FET GA618082). We gratefully acknowledge the computing resources provided on Blues and Fusion, high-performance computing clusters operated by the Laboratory Computing Resource Center at Argonne National Laboratory. NR 40 TC 4 Z9 4 U1 12 U2 54 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAR 31 PY 2015 VL 91 IS 11 AR 115143 DI 10.1103/PhysRevB.91.115143 PG 8 WC Physics, Condensed Matter SC Physics GA CE7ZP UT WOS:000352060800002 ER PT J AU Akopov, N Akopov, Z Augustyniak, W Avakian, R Avetissian, A Avetisyan, E Belostotski, S Blok, HP Borissov, A Bowles, J Bryzgalov, V Burns, J Capitani, GP Cisbani, E Ciullo, G Contalbrigo, M Dalpiaz, PF Deconinck, W De Leo, R De Sanctis, E Di Nezza, P Elbakian, G Etzelmuller, E Fabbri, R Fantoni, A Felawka, L Frullani, S Gabbert, D Garcia, JG Garibaldi, F Gavrilov, G Giordano, F Gliske, S Hartig, M Hasch, D Holler, Y Hristova, I Imazu, Y Ivanilov, A Jackson, HE Joosten, S Kaiser, R Karyan, G Keri, T Kinney, E Kisselev, A Kozlov, V Kravchenko, P Krivokhijine, VG Lagamba, L Lapikas, L Lehmann, I Ruiz, AL Lorenzon, W Lu, X Ma, BQ Mahon, D Manaenkov, SI Mao, Y Marianski, B de la Ossa, AM Marukyan, H Miller, CA Miyachi, Y Movsisyan, A Murray, M Nappi, E Nass, A Negodaev, M Nowak, WD Pappalardo, LL Perez-Benito, R Petrosyan, A Reimer, PE Reolon, AR Riedl, C Rith, K Rosner, G Rostomyan, A Rubin, J Ryckbosch, D Salomatin, Y Schnell, G Schuler, KP Seitz, B Shibata, TA Stancari, M Steijger, JJM Taroian, S Terkulov, A Truty, R Trzcinski, A Tytgat, M Van Haarlem, Y Van Hulse, C Veretennikov, D Vikhrov, V Vilardi, I Wang, S Yaschenko, S Ye, H Ye, Z Yen, S Zihlmann, B Zupranski, P AF Akopov, N. Akopov, Z. Augustyniak, W. Avakian, R. Avetissian, A. Avetisyan, E. Belostotski, S. Blok, H. P. Borissov, A. Bowles, J. Bryzgalov, V. Burns, J. Capitani, G. P. Cisbani, E. Ciullo, G. Contalbrigo, M. Dalpiaz, P. F. Deconinck, W. De Leo, R. De Sanctis, E. Di Nezza, P. Elbakian, G. Etzelmueller, E. Fabbri, R. Fantoni, A. Felawka, L. Frullani, S. Gabbert, D. Garcia, J. Garay Garibaldi, F. Gavrilov, G. Giordano, F. Gliske, S. Hartig, M. Hasch, D. Holler, Y. Hristova, I. Imazu, Y. Ivanilov, A. Jackson, H. E. Joosten, S. Kaiser, R. Karyan, G. Keri, T. Kinney, E. Kisselev, A. Kozlov, V. Kravchenko, P. Krivokhijine, V. G. Lagamba, L. Lapikas, L. Lehmann, I. Ruiz, A. Lopez Lorenzon, W. Lu, X. Ma, B. -Q. Mahon, D. Manaenkov, S. I. Mao, Y. Marianski, B. de la Ossa, A. Martinez Marukyan, H. Miller, C. A. Miyachi, Y. Movsisyan, A. Murray, M. Nappi, E. Nass, A. Negodaev, M. Nowak, W. -D. Pappalardo, L. L. Perez-Benito, R. Petrosyan, A. Reimer, P. E. Reolon, A. R. Riedl, C. Rith, K. Rosner, G. Rostomyan, A. Rubin, J. Ryckbosch, D. Salomatin, Y. Schnell, G. Schueler, K. P. Seitz, B. Shibata, T. -A. Stancari, M. Steijger, J. J. M. Taroian, S. Terkulov, A. Truty, R. Trzcinski, A. Tytgat, M. Van Haarlem, Y. Van Hulse, C. Veretennikov, D. Vikhrov, V. Vilardi, I. Wang, S. Yaschenko, S. Ye, H. Ye, Z. Yen, S. Zihlmann, B. Zupranski, P. TI Pentaquark Theta(+) search at HERMES SO PHYSICAL REVIEW D LA English DT Article ID SKYRME MODEL; DECUPLET; BARYONS; RING AB The earlier search at HERMES for narrow baryon states excited in quasireal photoproduction, decaying through the channel pK(S)(0) -> p pi(+)pi(-), has been extended with improved decay-particle reconstruction, more advanced particle identification, and increased event samples. The structure observed earlier at an invariant mass of 1528 MeV shifts to 1522 MeV and the statistical significance drops to about 2 sigma for data taken with a deuterium target. The number of events above background is 68(-31)(+98)(stat) +/- 13(sys). No such structure is observed in the hydrogen data set. C1 [Jackson, H. E.; Reimer, P. E.; Rubin, J.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [De Leo, R.; Lagamba, L.; Nappi, E.; Vilardi, I.] Ist Nazl Fis Nucl, Sez Bari, I-70124 Bari, Italy. [Ma, B. -Q.; Mao, Y.; Wang, S.; Ye, H.] Peking Univ, Sch Phys, Beijing 100871, Peoples R China. [Garcia, J. Garay; Schnell, G.; Van Hulse, C.] Univ Basque Country, UPV EHU, Dept Theoret Phys, Bilbao 48080, Spain. [Garcia, J. Garay; Schnell, G.; Van Hulse, C.] Basque Fdn Sci, Ikerbasque, Bilbao 48013, Spain. [Kinney, E.; de la Ossa, A. Martinez] Univ Colorado, Nucl Phys Lab, Boulder, CO 80309 USA. [Akopov, Z.; Avetisyan, E.; Borissov, A.; Deconinck, W.; Garcia, J. Garay; Gavrilov, G.; Hartig, M.; Holler, Y.; de la Ossa, A. Martinez; Rostomyan, A.; Schueler, K. P.; Yaschenko, S.; Ye, Z.; Zihlmann, B.] DESY, D-22603 Hamburg, Germany. [Fabbri, R.; Gabbert, D.; Hristova, I.; Lu, X.; Negodaev, M.; Nowak, W. -D.; Riedl, C.] DESY, D-15738 Zeuthen, Germany. [Krivokhijine, V. G.] Joint Inst Nucl Res, Dubna 141980, Russia. [Kravchenko, P.; Nass, A.; Rith, K.; Yaschenko, S.] Univ Erlangen Nurnberg, Inst Phys, D-91058 Erlangen, Germany. [Ciullo, G.; Contalbrigo, M.; Dalpiaz, P. F.; Giordano, F.; Movsisyan, A.; Pappalardo, L. L.; Stancari, M.] Ist Nazl Fis Nucl, Sez Ferrara, I-44122 Ferrara, Italy. [Ciullo, G.; Contalbrigo, M.; Dalpiaz, P. F.; Giordano, F.; Movsisyan, A.; Pappalardo, L. L.; Stancari, M.] Univ Ferrara, Dipartimento Fis & Sci Terra, I-44122 Ferrara, Italy. [Capitani, G. P.; De Sanctis, E.; Di Nezza, P.; Fantoni, A.; Hasch, D.; Reolon, A. R.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Joosten, S.; Ruiz, A. Lopez; Ryckbosch, D.; Schnell, G.; Tytgat, M.; Van Haarlem, Y.; Van Hulse, C.] Univ Ghent, Dept Phys & Astron, B-9000 Ghent, Belgium. [Etzelmueller, E.; Keri, T.; Perez-Benito, R.] Univ Giessen, Phys Inst 2, D-35392 Giessen, Germany. [Bowles, J.; Burns, J.; Kaiser, R.; Keri, T.; Lehmann, I.; Mahon, D.; Murray, M.; Rosner, G.; Seitz, B.] Univ Glasgow, SUPA, Sch Phys & Astron, Glasgow G12 8QQ, Lanark, Scotland. [Giordano, F.; Joosten, S.; Riedl, C.; Rubin, J.; Truty, R.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Gliske, S.; Lorenzon, W.] Univ Michigan, Randall Lab Phys, Ann Arbor, MI 48109 USA. [Kozlov, V.; Terkulov, A.] Lebedev Phys Inst, Moscow 117924, Russia. [Lapikas, L.; Steijger, J. J. M.] Nikhef, Natl Inst Subat Phys, NL-1009 DB Amsterdam, Netherlands. [Belostotski, S.; Blok, H. P.; Gavrilov, G.; Kisselev, A.; Kravchenko, P.; Manaenkov, S. I.; Veretennikov, D.; Vikhrov, V.] BP Konstantinov Petersburg Nucl Phys Inst, Gatchina, Leningrad Regio, Russia. [Bryzgalov, V.; Ivanilov, A.; Salomatin, Y.] Inst High Energy Phys, Protvino 142281, Moscow Region, Russia. [Cisbani, E.; Frullani, S.; Garibaldi, F.] Ist Nazl Fis Nucl, Sez Roma, Grp Collegato Sanita, I-00161 Rome, Italy. [Cisbani, E.; Frullani, S.; Garibaldi, F.] Ist Super Sanita, I-00161 Rome, Italy. [Felawka, L.; Gavrilov, G.; Miller, C. A.; Yen, S.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Imazu, Y.; Miyachi, Y.; Shibata, T. -A.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [Blok, H. P.] Vrije Univ Amsterdam, Dept Phys & Astron, NL-1081 HV Amsterdam, Netherlands. [Augustyniak, W.; Marianski, B.; Trzcinski, A.; Zupranski, P.] Natl Ctr Nucl Res, PL-00689 Warsaw, Poland. [Akopov, N.; Avakian, R.; Avetissian, A.; Elbakian, G.; Karyan, G.; Marukyan, H.; Movsisyan, A.; Petrosyan, A.; Taroian, S.] Yerevan Phys Inst, Yerevan 375036, Armenia. RP Akopov, N (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Cisbani, Evaristo/C-9249-2011; Kozlov, Valentin/M-8000-2015; Negodaev, Mikhail/A-7026-2014; Terkulov, Adel/M-8581-2015 OI Cisbani, Evaristo/0000-0002-6774-8473; FU DESY management FX We gratefully acknowledge the DESY management for its support, the staff at DESY and the collaborating institutions for their significant effort, as well as our national funding agencies for financial support. NR 20 TC 0 Z9 0 U1 1 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD MAR 31 PY 2015 VL 91 IS 5 AR 057101 DI 10.1103/PhysRevD.91.057101 PG 5 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CE8AF UT WOS:000352062400003 ER PT J AU Lees, JP Poireau, V Tisserand, V Grauges, E Palano, A Eigen, G Stugu, B Brown, DN Kerth, LT Kolomensky, YG Lee, MJ Lynch, G Koch, H Schroeder, T Hearty, C Mattison, TS McKenna, JA So, RY Khan, A Blinov, VE Buzykaev, AR Druzhinin, VP Golubev, VB Kravchenko, EA Onuchin, AP Serednyakov, SI Skovpen, YI Solodov, EP Todyshev, KY Lankford, AJ Mandelkern, M Dey, B Gary, JW Long, O Campagnari, C Sevilla, MF Hong, TM Kovalskyi, D Richman, JD West, CA Eisner, AM Lockman, WS Vazquez, WP Schumm, BA Seiden, A Chao, DS Cheng, CH Echenard, B Flood, KT Hitlin, DG Miyashita, TS Ongmongkolkul, P Porter, FC Rohrken, M Andreassen, R Huard, Z Meadows, BT Pushpawela, BG Sokoloff, MD Sun, L Bloom, PC Ford, WT Gaz, A Smith, JG Wagner, SR Ayad, R Toki, WH Spaan, B Bernard, D Verderi, M Playfer, S Bettoni, D Bozzi, C Calabrese, R Cibinetto, G Fioravanti, E Garzia, I Luppi, E Piemontese, L Santoro, V Calcaterra, A De Sangro, R Finocchiaro, G Martellotti, S Patteri, P Peruzzi, IM Piccolo, M Rama, M Zallo, A Contri, R Lo Vetere, M Monge, MR Passaggio, S Patrignani, C Robutti, E Bhuyan, B Prasad, V Adametz, A Uwer, U Lacker, HM Dauncey, PD Mallik, U Chen, C Cochran, J Prell, S Ahmed, H Gritsan, AV Arnaud, N Davier, M Derkach, D Grosdidier, G Le Diberder, F Lutz, AM Malaescu, B Roudeau, P Stocchi, A Wormser, G Lange, DJ Wright, DM Coleman, JP Fry, JR Gabathuler, E Hutchcroft, DE Payne, DJ Touramanis, C Bevan, AJ Di Lodovico, F Sacco, R Cowan, G Bougher, J Brown, DN Davis, CL Denig, AG Fritsch, M Gradl, W Griessinger, K Hafner, A Schubert, KR Barlow, RJ Lafferty, GD Cenci, R Hamilton, B Jawahery, A Roberts, DA Cowan, R Sciolla, G Cheaib, R Patel, PM Robertson, SH Neri, N Palombo, F Cremaldi, L Godang, R Sonnek, P Summers, DJ Simard, M Taras, P De Nardo, G Onorato, G Sciacca, C Martinelli, M Raven, G Jessop, CP LoSecco, JM Honscheid, K Kass, R Feltresi, E Margoni, M Morandin, M Posocco, M Rotondo, M Simi, G Simonetto, F Stroili, R Akar, S Ben-Haim, E Bomben, M Bonneaud, GR Briand, H Calderini, G Chauveau, J Leruste, P Marchiori, G Ocariz, J Biasini, M Manoni, E Pacetti, S Rossi, A Angelini, C Batignani, G Bettarini, S Carpinelli, M Casarosa, G Cervelli, A Chrzaszcz, M Forti, F Giorgi, MA Lusiani, A Oberhof, B Paoloni, E Perez, A Rizzo, G Walsh, JJ Pegna, DL Olsen, J Smith, AJS Faccini, R Ferrarotto, F Ferroni, F Gaspero, M Gioi, LL Pilloni, A Piredda, G Bunger, C Dittrich, S Grunberg, O Hess, M Leddig, T Voss, C Waldi, R Adye, T Olaiya, EO Wilson, FF Emery, S Vasseur, G Anulli, F Aston, D Bard, DJ Cartaro, C Convery, MR Dorfan, J Dubois-Felsmann, GP Dunwoodie, W Ebert, M Field, RC Fulsom, BG Graham, MT Hast, C Innes, WR Kim, P Leith, DWGS Lewis, P Lindemann, D Luitz, S Luth, V Lynch, HL MacFarlane, DB Muller, DR Neal, H Perl, M Pulliam, T Ratcliff, BN Roodman, A Salnikov, AA Schindler, RH Snyder, A Su, D Sullivan, MK Va'vra, J Wisniewski, WJ Wulsin, HW Purohit, MV White, RM Wilson, JR Randle-Conde, A Sekula, SJ Bellis, M Burchat, PR Puccio, EMT Alam, MS Ernst, JA Gorodeisky, R Guttman, N Peimer, DR Soffer, A Spanier, SM Ritchie, JL Ruland, AM Schwitters, RF Wray, BC Izen, JM Lou, XC Bianchi, F De Mori, F Filippi, A Gamba, D Lanceri, L Vitale, L Martinez-Vidal, F Oyanguren, A Villanueva-Perez, P Albert, J Banerjee, S Beaulieu, A Bernlochner, FU King, HHFCGJ King, GJ Kowalewski, R Lewczuk, MJ Lueck, T Nugent, IM Roney, JM Sobie, RJ Tasneem, N Gershon, TJ Harrison, PF Latham, TE Band, HR Dasu, S Pan, Y Prepost, R Wu, SL AF Lees, J. P. Poireau, V. Tisserand, V. Grauges, E. Palano, A. Eigen, G. Stugu, B. Brown, D. N. Kerth, L. T. Kolomensky, Yu. G. Lee, M. J. Lynch, G. Koch, H. Schroeder, T. Hearty, C. Mattison, T. S. McKenna, J. A. So, R. Y. Khan, A. Blinov, V. E. Buzykaev, A. R. Druzhinin, V. P. Golubev, V. B. Kravchenko, E. A. Onuchin, A. P. Serednyakov, S. I. Skovpen, Yu. I. Solodov, E. P. Todyshev, K. Yu. Lankford, A. J. Mandelkern, M. Dey, B. Gary, J. W. Long, O. Campagnari, C. Sevilla, M. Franco Hong, T. M. Kovalskyi, D. Richman, J. D. West, C. A. Eisner, A. M. Lockman, W. S. Vazquez, W. Panduro Schumm, B. A. Seiden, A. Chao, D. S. Cheng, C. H. Echenard, B. Flood, K. T. Hitlin, D. G. Miyashita, T. S. Ongmongkolkul, P. Porter, F. C. Roehrken, M. Andreassen, R. Huard, Z. Meadows, B. T. Pushpawela, B. G. Sokoloff, M. D. Sun, L. Bloom, P. C. Ford, W. T. Gaz, A. Smith, J. G. Wagner, S. R. Ayad, R. Toki, W. H. Spaan, B. Bernard, D. Verderi, M. Playfer, S. Bettoni, D. Bozzi, C. Calabrese, R. Cibinetto, G. Fioravanti, E. Garzia, I. Luppi, E. Piemontese, L. Santoro, V. Calcaterra, A. De Sangro, R. Finocchiaro, G. Martellotti, S. Patteri, P. Peruzzi, I. M. Piccolo, M. Rama, M. Zallo, A. Contri, R. Lo Vetere, M. Monge, M. R. Passaggio, S. Patrignani, C. Robutti, E. Bhuyan, B. Prasad, V. Adametz, A. Uwer, U. Lacker, H. M. Dauncey, P. D. Mallik, U. Chen, C. Cochran, J. Prell, S. Ahmed, H. Gritsan, A. V. Arnaud, N. Davier, M. Derkach, D. Grosdidier, G. Le Diberder, F. Lutz, A. M. Malaescu, B. Roudeau, P. Stocchi, A. Wormser, G. Lange, D. J. Wright, D. M. Coleman, J. P. Fry, J. R. Gabathuler, E. Hutchcroft, D. E. Payne, D. J. Touramanis, C. Bevan, A. J. Di Lodovico, F. Sacco, R. Cowan, G. Bougher, J. Brown, D. N. Davis, C. L. Denig, A. G. Fritsch, M. Gradl, W. Griessinger, K. Hafner, A. Schubert, K. R. Barlow, R. J. Lafferty, G. D. Cenci, R. Hamilton, B. Jawahery, A. Roberts, D. A. Cowan, R. Sciolla, G. Cheaib, R. Patel, P. M. Robertson, S. H. Neri, N. Palombo, F. Cremaldi, L. Godang, R. Sonnek, P. Summers, D. J. Simard, M. Taras, P. De Nardo, G. Onorato, G. Sciacca, C. Martinelli, M. Raven, G. Jessop, C. P. LoSecco, J. M. Honscheid, K. Kass, R. Feltresi, E. Margoni, M. Morandin, M. Posocco, M. Rotondo, M. Simi, G. Simonetto, F. Stroili, R. Akar, S. Ben-Haim, E. Bomben, M. Bonneaud, G. R. Briand, H. Calderini, G. Chauveau, J. Leruste, Ph. Marchiori, G. Ocariz, J. Biasini, M. Manoni, E. Pacetti, S. Rossi, A. Angelini, C. Batignani, G. Bettarini, S. Carpinelli, M. Casarosa, G. Cervelli, A. Chrzaszcz, M. Forti, F. Giorgi, M. A. Lusiani, A. Oberhof, B. Paoloni, E. Perez, A. Rizzo, G. Walsh, J. J. Pegna, D. Lopes Olsen, J. Smith, A. J. S. Faccini, R. Ferrarotto, F. Ferroni, F. Gaspero, M. Gioi, L. Li Pilloni, A. Piredda, G. Buenger, C. Dittrich, S. Gruenberg, O. Hess, M. Leddig, T. Voss, C. Waldi, R. Adye, T. Olaiya, E. O. Wilson, F. F. Emery, S. Vasseur, G. Anulli, F. Aston, D. Bard, D. J. Cartaro, C. Convery, M. R. Dorfan, J. Dubois-Felsmann, G. P. Dunwoodie, W. Ebert, M. Field, R. C. Fulsom, B. G. Graham, M. T. Hast, C. Innes, W. R. Kim, P. Leith, D. W. G. S. Lewis, P. Lindemann, D. Luitz, S. Luth, V. Lynch, H. L. MacFarlane, D. B. Muller, D. R. Neal, H. Perl, M. Pulliam, T. Ratcliff, B. N. Roodman, A. Salnikov, A. A. Schindler, R. H. Snyder, A. Su, D. Sullivan, M. K. Va'vra, J. Wisniewski, W. J. Wulsin, H. W. Purohit, M. V. White, R. M. Wilson, J. R. Randle-Conde, A. Sekula, S. J. Bellis, M. Burchat, P. R. Puccio, E. M. T. Alam, M. S. Ernst, J. A. Gorodeisky, R. Guttman, N. Peimer, D. R. Soffer, A. Spanier, S. M. Ritchie, J. L. Ruland, A. M. Schwitters, R. F. Wray, B. C. Izen, J. M. Lou, X. C. Bianchi, F. De Mori, F. Filippi, A. Gamba, D. Lanceri, L. Vitale, L. Martinez-Vidal, F. Oyanguren, A. Villanueva-Perez, P. Albert, J. Banerjee, Sw. Beaulieu, A. Bernlochner, F. U. Choi, H. H. F. King, G. J. Kowalewski, R. Lewczuk, M. J. Lueck, T. Nugent, I. M. Roney, J. M. Sobie, R. J. Tasneem, N. Gershon, T. J. Harrison, P. F. Latham, T. E. Band, H. R. Dasu, S. Pan, Y. Prepost, R. Wu, S. L. TI Measurement of the D-0 -> pi(-)e(+)nu(e) differential decay branching fraction as a function of q(2) and study of form factor parametrizations SO PHYSICAL REVIEW D LA English DT Article ID SEMILEPTONIC DECAYS; BABAR DETECTOR; MESON DECAYS; RADIATIVE-CORRECTIONS; QUARK-MODEL; HEAVY; CHROMODYNAMICS; PHYSICS; SHAPES AB Based on a sample of 500 million e(+)e(-) -> c (c) over bar events recorded by the BABAR detector at c. m. energies of close to 10.6 GeV, we report on a study of the decay D0 ->pi(-)e(+)nu(e). We measure the ratio of branching fractions, R-D = B(D-0 -> pi(-)e(+)nu(e))/beta(D-0 -> K-pi(+)) = 0.0713 +/- 0.0017(stat) +/- 0.0024(syst), and use the present world average for B(D-0 -> K-pi(+)) to obtain B(D-0 -> pi(-)e(+)nu e) = (2.770 +/- 0.068(stat) +/- 0.092(syst) +/- 0.037(ext)) x 10(-3) where the third error accounts for the uncertainty on the branching fraction for the reference channel. The measured dependence of the differential branching fraction on q(2), the four-momentum transfer squared between the D and the pi meson, is compared to various theoretical predictions for the hadronic form factor, f(+,D)(pi)(q(2)), and the normalization vertical bar V-cd vertical bar x f(+,D)(pi)(q(2) = 0) = 0.1374 +/- 0.0038(stat) +/- 0.0022(sys)t +/- 0.0009(ext). is extracted from a fit to data. Using the most recent LQCD prediction of f(+,D)(pi)(q(2) = 0) = 0.666 +/- 0.029, we obtain vertical bar V-cd vertical bar = 0.206 +/- 0.007(exp) +/- 0.009(LQCD). Assuming, instead, vertical bar V-cd vertical bar = vertical bar V-us vertical bar = 0.2252 +/- 0.0009, we obtain f(+,D)(pi)(q(2) = 0) = 0.610 +/- 0.020(exp) +/- 0.005(ext). The q(2) dependence of f(+,D)(pi)(q(2)) is compared to a variety of multipole parametrizations. 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R.; Briand, H.; Calderini, G.; Chauveau, J.; Leruste, Ph.; Marchiori, G.; Ocariz, J.] Univ Paris 07, Univ Paris 06, IN2P3 CNRS, Lab Phys Nucl & Hautes Energies, F-75252 Paris, France. [Biasini, M.; Manoni, E.; Pacetti, S.; Rossi, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06123 Perugia, Italy. [Ayad, R.; Peruzzi, I. M.; Adametz, A.; Biasini, M.; Pacetti, S.; Anulli, F.] Univ Perugia, Dipartimento Fis, I-06123 Perugia, Italy. [Angelini, C.; Batignani, G.; Bettarini, S.; Carpinelli, M.; Casarosa, G.; Cervelli, A.; Chrzaszcz, M.; Forti, F.; Giorgi, M. A.; Lusiani, A.; Oberhof, B.; Paoloni, E.; Perez, A.; Rizzo, G.; Walsh, J. J.] Ist Nazl Fis Nucl, Sez Pisa, I-56127 Pisa, Italy. [Angelini, C.; Batignani, G.; Bettarini, S.; Carpinelli, M.; Casarosa, G.; Cervelli, A.; Forti, F.; Giorgi, M. A.; Oberhof, B.; Paoloni, E.; Rizzo, G.] Univ Pisa, Dipartimento Fis, I-56127 Pisa, Italy. [Lusiani, A.] Scuola Normale Super Pisa, I-56127 Pisa, Italy. [Pegna, D. Lopes; Olsen, J.; Smith, A. J. S.] Princeton Univ, Princeton, NJ 08544 USA. [Faccini, R.; Ferrarotto, F.; Ferroni, F.; Gaspero, M.; Gioi, L. Li; Pilloni, A.; Piredda, G.; White, R. M.] Ist Nazl Fis Nucl, Sez Roma, I-00185 Rome, Italy. [Faccini, R.; Ferroni, F.; Gaspero, M.; Pilloni, A.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Buenger, C.; Dittrich, S.; Gruenberg, O.; Hess, M.; Leddig, T.; Voss, C.; Waldi, R.] Univ Rostock, D-18051 Rostock, Germany. [Adye, T.; Olaiya, E. O.; Wilson, F. F.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Emery, S.; Vasseur, G.] CEA, Irfu, SPP, Ctr Saclay, F-91191 Gif Sur Yvette, France. [Anulli, F.; Aston, D.; Bard, D. J.; Cartaro, C.; Convery, M. R.; Dorfan, J.; Dubois-Felsmann, G. P.; Dunwoodie, W.; Ebert, M.; Field, R. C.; Fulsom, B. G.; Graham, M. T.; Hast, C.; Innes, W. R.; Kim, P.; Leith, D. W. G. S.; Lewis, P.; Lindemann, D.; Luitz, S.; Luth, V.; Lynch, H. L.; MacFarlane, D. B.; Muller, D. R.; Neal, H.; Perl, M.; Pulliam, T.; Ratcliff, B. N.; Roodman, A.; Salnikov, A. A.; Schindler, R. H.; Snyder, A.; Su, D.; Sullivan, M. K.; Va'vra, J.; Wisniewski, W. J.; Wulsin, H. W.] SLAC Natl Accelerator Lab, Stanford, CA 94309 USA. [Purohit, M. V.; White, R. M.; Wilson, J. R.] Univ S Carolina, Columbia, SC 29208 USA. [Randle-Conde, A.; Sekula, S. J.] So Methodist Univ, Dallas, TX 75275 USA. [Bellis, M.; Burchat, P. R.; Puccio, E. M. T.] Stanford Univ, Stanford, CA 94305 USA. [Alam, M. S.; Ernst, J. A.] SUNY Albany, Albany, NY 12222 USA. [Gorodeisky, R.; Guttman, N.; Peimer, D. R.; Soffer, A.] Tel Aviv Univ, Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Spanier, S. M.] Univ Tennessee, Knoxville, TN 37996 USA. [Ritchie, J. L.; Ruland, A. M.; Schwitters, R. F.; Wray, B. C.] Univ Texas Austin, Austin, TX 78712 USA. [Izen, J. M.; Lou, X. C.] Univ Texas Dallas, Richardson, TX 75083 USA. [Bianchi, F.; De Mori, F.; Filippi, A.; Gamba, D.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Bianchi, F.; De Mori, F.; Gamba, D.] Univ Turin, Dipartimento Fis, I-10125 Turin, Italy. [Lanceri, L.; Vitale, L.] Ist Nazl Fis Nucl, Sez Trieste, I-34127 Trieste, Italy. [Lanceri, L.; Vitale, L.] Univ Trieste, Dipartmento Fis, I-34127 Trieste, Italy. [Martinez-Vidal, F.; Oyanguren, A.; Villanueva-Perez, P.] Univ Valencia, CSIC, IFIC, E-46071 Valencia, Spain. [Albert, J.; Banerjee, Sw.; Beaulieu, A.; Bernlochner, F. U.; Choi, H. H. F.; King, G. J.; Kowalewski, R.; Lewczuk, M. J.; Lueck, T.; Nugent, I. M.; Roney, J. M.; Sobie, R. J.; Tasneem, N.] Univ Victoria, Victoria, BC V8W 3P6, Canada. [Gershon, T. J.; Harrison, P. F.; Latham, T. E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Band, H. R.; Dasu, S.; Pan, Y.; Prepost, R.; Wu, S. L.] Univ Wisconsin, Madison, WI 53706 USA. [Carpinelli, M.] Univ Sassari, I-07100 Sassari, Italy. RP Lees, JP (reprint author), Univ Savoie, CNRS, IN2P3, LAPP, F-74941 Annecy Le Vieux, France. RI Morandin, Mauro/A-3308-2016; Lusiani, Alberto/A-3329-2016; Di Lodovico, Francesca/L-9109-2016; Calcaterra, Alessandro/P-5260-2015; Oyanguren, Arantza/K-6454-2014; Monge, Maria Roberta/G-9127-2012; Lo Vetere, Maurizio/J-5049-2012; White, Ryan/E-2979-2015; Kravchenko, Evgeniy/F-5457-2015; Lusiani, Alberto/N-2976-2015; Forti, Francesco/H-3035-2011; Patrignani, Claudia/C-5223-2009; Luppi, Eleonora/A-4902-2015; Calabrese, Roberto/G-4405-2015; Kolomensky, Yury/I-3510-2015; Martinez Vidal, F*/L-7563-2014 OI Morandin, Mauro/0000-0003-4708-4240; Lusiani, Alberto/0000-0002-6876-3288; Di Lodovico, Francesca/0000-0003-3952-2175; Calcaterra, Alessandro/0000-0003-2670-4826; Oyanguren, Arantza/0000-0002-8240-7300; Monge, Maria Roberta/0000-0003-1633-3195; Lo Vetere, Maurizio/0000-0002-6520-4480; White, Ryan/0000-0003-3589-5900; Lusiani, Alberto/0000-0002-6876-3288; Forti, Francesco/0000-0001-6535-7965; Patrignani, Claudia/0000-0002-5882-1747; Luppi, Eleonora/0000-0002-1072-5633; Calabrese, Roberto/0000-0002-1354-5400; Kolomensky, Yury/0000-0001-8496-9975; Martinez Vidal, F*/0000-0001-6841-6035 FU US Department of Energy and National Science Foundation; Natural Sciences and Engineering Research Council (Canada); Commissariat a l'Energie Atomique (France); Institut National de Physique Nucleaire et de Physique des Particules (France); Bundesministerium fur Bildung und Forschung (Germany); Deutsche Forschungsgemeinschaft (Germany); Istituto Nazionale di Fisica Nucleare (Italy); Foundation for Fundamental Research on Matter (The Netherlands); Research Council of Norway; Ministry of Education and Science of the Russian Federation, Ministerio de Economia y Competitividad (Spain); Science and Technology Facilities Council (United Kingdom); Binational Science Foundation (U.S.-Israel); Marie-Curie IEF program (European Union); A. P. Sloan Foundation (USA) FX The authors wish to thank D. Becirevic, S. Descotes-Genon, and A. Le Yaouanc for their help with the theoretical interpretation of these results. We are grateful for the extraordinary contributions of our PEP-II colleagues in achieving the excellent luminosity and machine conditions that have made this work possible. The success of this project also relies critically on the expertise and dedication of the computing organizations that support BABAR. The collaborating institutions wish to thank SLAC for its support and the kind hospitality extended to them. This work is supported by the US Department of Energy and National Science Foundation, the Natural Sciences and Engineering Research Council (Canada), the Commissariat a l'Energie Atomique and Institut National de Physique Nucleaire et de Physique des Particules (France), the Bundesministerium fur Bildung und Forschung and Deutsche Forschungsgemeinschaft (Germany), the Istituto Nazionale di Fisica Nucleare (Italy), the Foundation for Fundamental Research on Matter (The Netherlands), the Research Council of Norway, the Ministry of Education and Science of the Russian Federation, Ministerio de Economia y Competitividad (Spain), the Science and Technology Facilities Council (United Kingdom), and the Binational Science Foundation (U.S.-Israel). Individuals have received support from the Marie-Curie IEF program (European Union) and the A. P. Sloan Foundation (USA). NR 59 TC 4 Z9 5 U1 1 U2 15 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD MAR 31 PY 2015 VL 91 IS 5 AR 052022 DI 10.1103/PhysRevD.91.052022 PG 25 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CE8AF UT WOS:000352062400001 ER PT J AU Adams, BW Kim, KJ AF Adams, B. W. Kim, K. -J. TI X-ray comb generation from nuclear-resonance-stabilized x-ray free-electron laser oscillator for fundamental physics and precision metrology SO PHYSICAL REVIEW SPECIAL TOPICS-ACCELERATORS AND BEAMS LA English DT Article ID QUANTUM AB An x-ray free-electron laser oscillator (XFELO) is a next-generation x-ray source, similar to free-electron laser oscillators at VUV and longer wavelengths but using crystals as high-reflectivity x-ray mirrors. Each output pulse from an XFELO is fully coherent with high spectral purity. The temporal coherence length can further be increased drastically, from picoseconds to microseconds or even longer, by phase-locking successive XFELO output pulses, using the narrow nuclear resonance lines of nuclei such as Fe-57 as a reference. We show that the phase fluctuation due to the seismic activities is controllable and that due to spontaneous emission is small. The fluctuation of electron-bunch spacing contributes mainly to the envelope fluctuation but not to the phase fluctuation. By counting the number of standing-wave maxima formed by the output of the nuclear-resonance-stabilized (NRS) XFELO over an optically known length, the wavelength of the nuclear resonance can be accurately measured, possibly leading to a new length or frequency standard at x-ray wavelengths. A NRS-XFELO will be an ideal source for experimental x-ray quantum optics as well as other fundamental physics. The technique can be refined for other, narrower resonances such as Ta-181 or Sc-45. C1 [Adams, B. W.; Kim, K. -J.] Argonne Natl Lab, Lemont, IL 60439 USA. RP Adams, BW (reprint author), Argonne Natl Lab, 9700 South Cass Ave, Lemont, IL 60439 USA. FU U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX We thank Jorg Evers for helpful discussions on quantum-optical applications of the XFELO. This work was supported by the U.S. Department of Energy, Office of Basic Energy Sciences under Contract No. DE-AC02-06CH11357. NR 32 TC 1 Z9 1 U1 1 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-4402 J9 PHYS REV SPEC TOP-AC JI Phys. Rev. Spec. Top.-Accel. Beams PD MAR 31 PY 2015 VL 18 IS 3 AR 030711 DI 10.1103/PhysRevSTAB.18.030711 PG 11 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA CE8EK UT WOS:000352074100001 ER PT J AU Bartsch, MS Edwards, HS Lee, D Moseley, CE Tew, KE Renzi, RF Van de Vreugde, JL Kim, H Knight, DL Sinha, A Branda, SS Patel, KD AF Bartsch, Michael S. Edwards, Harrison S. Lee, Daniel Moseley, Caroline E. Tew, Karen E. Renzi, Ronald F. Van de Vreugde, James L. Kim, Hanyoup Knight, Daniel L. Sinha, Anupama Branda, Steven S. Patel, Kamlesh D. TI The Rotary Zone Thermal Cycler: A Low-Power System Enabling Automated Rapid PCR SO PLOS ONE LA English DT Article ID POLYMERASE-CHAIN-REACTION; NUCLEIC-ACID AMPLIFICATION; FORENSIC DNA ANALYSIS; REAL-TIME PCR; DIGITAL MICROFLUIDIC PLATFORM; OF-CARE DIAGNOSTICS; ON-A-CHIP; CAPILLARY ELECTROPHORESIS MICROSYSTEM; FLOW-THROUGH PCR; GENETIC-ANALYSIS AB Advances in molecular biology, microfluidics, and laboratory automation continue to expand the accessibility and applicability of these methods beyond the confines of conventional, centralized laboratory facilities and into point of use roles in clinical, military, forensic, and field-deployed applications. As a result, there is a growing need to adapt the unit operations of molecular biology (e.g., aliquoting, centrifuging, mixing, and thermal cycling) to compact, portable, low-power, and automation-ready formats. Here we present one such adaptation, the rotary zone thermal cycler (RZTC), a novel wheel-based device capable of cycling up to four different fixed-temperature blocks into contact with a stationary 4-microliter capillary-bound sample to realize 1-3 second transitions with steady state heater power of less than 10 W. We demonstrate the utility of the RZTC for DNA amplification as part of a highly integrated rotary zone PCR (rzPCR) system that uses low-volume valves and syringe-based fluid handling to automate sample loading and unloading, thermal cycling, and between-run cleaning functionalities in a compact, modular form factor. In addition to characterizing the performance of the RZTC and the efficacy of different online cleaning protocols, we present preliminary results for rapid single-plex PCR, multiplex short tandem repeat (STR) amplification, and second strand cDNA synthesis. C1 [Bartsch, Michael S.; Edwards, Harrison S.; Lee, Daniel; Moseley, Caroline E.; Tew, Karen E.; Renzi, Ronald F.; Van de Vreugde, James L.; Kim, Hanyoup; Sinha, Anupama; Branda, Steven S.; Patel, Kamlesh D.] Sandia Natl Labs, Livermore, CA 94550 USA. [Knight, Daniel L.] SequoiaTek Corp, Logan, UT USA. RP Bartsch, MS (reprint author), Sandia Natl Labs, Livermore, CA 94550 USA. EM mbarts@sandia.gov FU U.S. Department of Defense Rapid Reaction Technology Office on behalf of the U.S. Army Criminal Investigation Laboratory; Sandia National Laboratories internal Laboratory Directed Research and Development grants; Department of Homeland Security HS-STEM internship program; United States Department of Energy [DE-AC04-94AL85000] FX This work was funded in part by the U.S. Department of Defense Rapid Reaction Technology Office on behalf of the U.S. Army Criminal Investigation Laboratory as part of the Battlefield Automated DNA Analysis and Sampling System project. Additional support was provided by Sandia National Laboratories internal Laboratory Directed Research and Development grants. Support for Harrison Edwards, Daniel Lee, Caroline Moseley, and Karen Tew was provided by the Department of Homeland Security HS-STEM internship program. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy under Contract DE-AC04-94AL85000. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 153 TC 1 Z9 1 U1 4 U2 33 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAR 31 PY 2015 VL 10 IS 3 AR UNSP e0118182 DI 10.1371/journal.pone.0118182 PG 35 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CE8IF UT WOS:000352084800003 PM 25826708 ER PT J AU Jones, SR Wilson, TD Brown, ME Rahn-Lee, L Yu, Y Fredriksen, LL Ozyamak, E Komeili, A Chang, MCY AF Jones, Stephanie R. Wilson, Tiffany D. Brown, Margaret E. Rahn-Lee, Lilah Yu, Yi Fredriksen, Laura L. Ozyamak, Ertan Komeili, Arash Chang, Michelle C. Y. TI Genetic and biochemical investigations of the role of MamP in redox control of iron biomineralization in Magnetospirillum magneticum SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE biomineralization; iron; magnetosome; cytochrome; MamP ID C-TYPE CYTOCHROME; MAGNETOSOME FORMATION; ESCHERICHIA-COLI; CRYSTAL-GROWTH; PROTEIN; OXIDATION; BACTERIA; GRYPHISWALDENSE; MINERALIZATION; FERROOXIDANS AB Magnetotactic bacteria have evolved complex subcellular machinery to construct linear chains of magnetite nanocrystals that allow the host cell to sense direction. Each mixed-valent iron nanoparticle is mineralized from soluble iron within a membrane-encapsulated vesicle termed the magnetosome, which serves as a specialized compartment that regulates the iron, redox, and pH environment of the growing mineral. To dissect the biological components that control this process, we have carried out a genetic and biochemical study of proteins proposed to function in iron mineralization. In this study, we show that the redox sites of c-type cytochromes of the Magnetospirillum magneticum AMB-1 magnetosome island, MamP and MamT, are essential to their physiological function and that ablation of one or both heme motifs leads to loss of function, suggesting that their ability to carry out redox chemistry in vivo is important. We also develop a method to heterologously express fully heme-loaded MamP from AMB-1 for in vitro biochemical studies, which show that its Fe(III)-Fe(II) redox couple is set at an unusual potential (-89 +/- 11 mV) compared with other related cytochromes involved in iron reduction or oxidation. Despite its low reduction potential, it remains competent to oxidize Fe(II) to Fe(III) and mineralize iron to produce mixed-valent iron oxides. Finally, in vitro mineralization experiments suggest that Mms mineral-templating peptides from AMB-1 can modulate the iron redox chemistry of MamP. C1 [Jones, Stephanie R.; Wilson, Tiffany D.; Brown, Margaret E.; Yu, Yi; Fredriksen, Laura L.; Chang, Michelle C. Y.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Rahn-Lee, Lilah; Ozyamak, Ertan; Komeili, Arash] Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. [Komeili, Arash; Chang, Michelle C. Y.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Chang, Michelle C. Y.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Chang, MCY (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM mcchang@berkeley.edu OI Fredriksen, Laura/0000-0002-1987-1549 FU Office of Basic Energy Sciences of the Department of Energy [DE-AC02-05CH11231]; Defense Advanced Research Projects Agency [N66001-12-1-4230]; NIH [1 T32 GMO66698, R01GM084122, S10RR025622]; NSF; Office of Naval Research [N000141310421] FX We thank Prof. Peidong Yang for assistance with HRTEM using the National Center for Electron Microscopy at Lawrence Berkeley National Laboratory, supported by the Office of Basic Energy Sciences of the Department of Energy (DE-AC02-05CH11231). This work was funded by generous support from the Defense Advanced Research Projects Agency (N66001-12-1-4230). S.R.J. and L.L.F. also acknowledge the support of NIH Training Grant (1 T32 GMO66698) and NSF Graduate Research Fellowships. A.K. was supported by grants from NIH (R01GM084122) and the Office of Naval Research (N000141310421). This work also used the Vincent J. Coates Proteomics/Mass Spectrometry Laboratory, supported in part by NIH S10RR025622. NR 32 TC 13 Z9 13 U1 2 U2 35 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAR 31 PY 2015 VL 112 IS 13 BP 3904 EP 3909 DI 10.1073/pnas.1417614112 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CE5ZH UT WOS:000351914500041 PM 25775527 ER PT J AU Mukherjee, S Huntemann, M Ivanova, N Kyrpides, NC Pati, A AF Mukherjee, Supratim Huntemann, Marcel Ivanova, Natalia Kyrpides, Nikos C. Pati, Amrita TI Large-scale contamination of microbial isolate genomes by Illumina PhiX control SO STANDARDS IN GENOMIC SCIENCES LA English DT Editorial Material DE Next-generation sequencing; PhiX; Contamination; Comparative genomics ID ANNOTATION; ORGANISMS; PHYLOGENY; BACTERIA; SEQUENCE; PROPOSAL; ARCHAEA; SYSTEM AB With the rapid growth and development of sequencing technologies, genomes have become the new go-to for exploring solutions to some of the world's biggest challenges such as searching for alternative energy sources and exploration of genomic dark matter. However, progress in sequencing has been accompanied by its share of errors that can occur during template or library preparation, sequencing, imaging or data analysis. In this study we screened over 18,000 publicly available microbial isolate genome sequences in the Integrated Microbial Genomes database and identified more than 1000 genomes that are contaminated with PhiX, a control frequently used during Illumina sequencing runs. Approximately 10% of these genomes have been published in literature and 129 contaminated genomes were sequenced under the Human Microbiome Project. Raw sequence reads are prone to contamination from various sources and are usually eliminated during downstream quality control steps. Detection of PhiX contaminated genomes indicates a lapse in either the application or effectiveness of proper quality control measures. The presence of PhiX contamination in several publicly available isolate genomes can result in additional errors when such data are used in comparative genomics analyses. Such contamination of public databases have far-reaching consequences in the form of erroneous data interpretation and analyses, and necessitates better measures to proofread raw sequences before releasing them to the broader scientific community. C1 [Mukherjee, Supratim; Huntemann, Marcel; Ivanova, Natalia; Kyrpides, Nikos C.; Pati, Amrita] DOE Joint Genome Inst, Walnut Creek, CA USA. [Ivanova, Natalia] King Abdulaziz Univ, Jeddah 21413, Saudi Arabia. RP Mukherjee, S (reprint author), DOE Joint Genome Inst, Walnut Creek, CA USA. EM supratimmukherjee@lbl.gov RI Kyrpides, Nikos/A-6305-2014; OI Kyrpides, Nikos/0000-0002-6131-0462; Ivanova, Natalia/0000-0002-5802-9485 NR 29 TC 11 Z9 11 U1 1 U2 4 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1944-3277 J9 STAND GENOMIC SCI JI Stand. Genomic Sci. PD MAR 30 PY 2015 VL 10 AR 18 DI 10.1186/1944-3277-10-18 PG 4 WC Genetics & Heredity; Microbiology SC Genetics & Heredity; Microbiology GA DA7LS UT WOS:000367986200001 PM 26203331 ER PT J AU Hambright, HG Meng, P Kumar, AP Ghosh, R AF Hambright, Heather G. Meng, Peng Kumar, Addanki P. Ghosh, Rita TI Inhibition of PI3K/AKT/mTOR axis disrupts oxidative stress-mediated survival of melanoma cells SO ONCOTARGET LA English DT Article DE Reactive oxygen species; oxidative stress; mTORC1; melanoma; Nexrutine(R) ID AMURENSE BARK EXTRACT; PROSTATE-CANCER; SIGNALING PATHWAY; TRANSGENIC ADENOCARCINOMA; METASTATIC MELANOMA; MALIGNANT-MELANOMA; PANCREATIC-CANCER; REDOX REGULATION; ACTIVATION; NEXRUTINE AB Elevated oxidative stress in cancer cells contributes to hyperactive proliferation and enhanced survival, which can be exploited using agents that increase reactive oxygen species (ROS) beyond a threshold level. Here we show that melanoma cells exhibit an oxidative stress phenotype compared with normal melanocytes, as evidenced by increased total cellular ROS, KEAP1/NRF2 pathway activity, protein damage, and elevated oxidized glutathione. Our overall objective was to test whether augmenting this high oxidative stress level in melanoma cells would inhibit their dependence on oncogenic PI3K/AKT/mTOR-mediated survival. We report that Nexrutine(R) augmented the constitutively elevated oxidative stress markers in melanoma cells, which was abrogated by N-acetyl cysteine (NAC) pre-treatment. Nexrutine(R) disrupted growth homeostasis by inhibiting proliferation, survival, and colony formation in melanoma cells without affecting melanocyte cell viability. Increased oxidative stress in melanoma cells inhibited PI3K/AKT/mTOR pathway through disruption of mTORC1 formation and phosphorylation of downstream targets p70S6K, 4EBP1 and rpS6. NAC pre-treatment reversed inhibition of mTORC1 targets, demonstrating a ROS-dependent mechanism. Overall, our results illustrate the importance of disruption of the intrinsically high oxidative stress in melanoma cells to selectively inhibit their survival mediated by PI3K/AKT/mTOR. C1 [Hambright, Heather G.; Meng, Peng; Kumar, Addanki P.; Ghosh, Rita] Univ Texas Hlth Sci Ctr San Antonio, Dept Urol, San Antonio, TX 78229 USA. [Kumar, Addanki P.; Ghosh, Rita] Univ Texas Hlth Sci Ctr San Antonio, Dept Pharmacol, San Antonio, TX 78229 USA. [Kumar, Addanki P.; Ghosh, Rita] Univ Texas Hlth Sci Ctr San Antonio, Dept Mol Med, San Antonio, TX 78229 USA. [Kumar, Addanki P.; Ghosh, Rita] Univ Texas Hlth Sci Ctr San Antonio, Canc Therapy & Res Ctr, San Antonio, TX 78229 USA. [Kumar, Addanki P.] South Texas Vet Hlth Care Syst, San Antonio, TX 78229 USA. [Meng, Peng] Lawrence Berkley Natl Lab, Div Life Sci, Berkeley, CA 94710 USA. RP Ghosh, R (reprint author), Univ Texas Hlth Sci Ctr San Antonio, Dept Urol, San Antonio, TX 78229 USA. EM ghoshr@uthscsa.edu FU VA Merit [I01BX000-766]; Cancer Therapy and Research Center at the University of Texas Health Science Center at San Antonio [2P30 CA054174-17]; [1R21CA125719] FX This work was funded in part by 1R21CA125719 (RG); VA Merit I01BX000-766 (APK); and through the Cancer Therapy and Research Center at the University of Texas Health Science Center at San Antonio (2P30 CA054174-17). NR 48 TC 16 Z9 17 U1 3 U2 7 PU IMPACT JOURNALS LLC PI ALBANY PA 6211 TIPTON HOUSE, STE 6, ALBANY, NY 12203 USA SN 1949-2553 J9 ONCOTARGET JI Oncotarget PD MAR 30 PY 2015 VL 6 IS 9 BP 7195 EP 7208 PG 14 WC Oncology; Cell Biology SC Oncology; Cell Biology GA CF8GI UT WOS:000352793800052 PM 25749517 ER PT J AU Adil, M Yang, S Mi, M Zhou, C Wang, JQ Zhang, R Liao, XQ Wang, Y Ren, XB Song, XP Ren, Y AF Adil, Murtaza Yang, Sen Mi, Meng Zhou, Chao Wang, Jieqiong Zhang, Rui Liao, Xiaoqi Wang, Yu Ren, Xiaobing Song, Xiaoping Ren, Yang TI Morphotropic phase boundary and magnetoelastic behaviour in ferromagnetic Tb1-xGdxFe2 system SO APPLIED PHYSICS LETTERS LA English DT Article ID SPIN-ORIENTATION; LAVES COMPOUNDS AB Morphotropic phase boundary (MPB), separating two ferroic phases of different crystal symmetries, has been studied extensively for its extraordinary enhancement of piezoelectricity in ferroelectrics. Based on the same mechanism, we have designed a magnetic MPB in the pseudobinary ferromagnetic system of Tb1-xGdxFe2 and the corresponding crystal structure, magnetic properties, and magnetostriction are explored. With the synchrotron x-ray diffractometry, the structure symmetry of TbFe2-rich compositions is detected to be rhombohedral (R) and that of GdFe2-rich compositions is tetragonal (T) below T-c. With the change of concentration, the value of magnetostriction of the samples changes monotonously, while the MPB composition Tb0.1Gd0.9Fe2, which corresponds to the coexistence of R and T phases, exhibits the maximum magnetization among all available compositions and superposition of magnetostriction behaviour of R and T phases. Our result of MPB phenomena in ferromagnets may provide an effective route to design functional magnetic materials with exotic properties. (C) 2015 AIP Publishing LLC. C1 [Adil, Murtaza; Yang, Sen; Mi, Meng; Zhou, Chao; Wang, Jieqiong; Zhang, Rui; Liao, Xiaoqi; Wang, Yu; Ren, Xiaobing; Song, Xiaoping] Xi An Jiao Tong Univ, Frontier Inst Sci & Technol, MOE Key Lab Nonequilibrium Synth & Modulat Conden, State Key Lab Mech Behav Mat,Sch Sci, Xian 710049, Peoples R China. [Ren, Yang] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. RP Adil, M (reprint author), Xi An Jiao Tong Univ, Frontier Inst Sci & Technol, MOE Key Lab Nonequilibrium Synth & Modulat Conden, State Key Lab Mech Behav Mat,Sch Sci, Xian 710049, Peoples R China. EM yang.sen@mail.xjtu.edu.cn; zhouch1982@gmail.com; xpsong@mail.xjtu.edu.cn RI Yang, Sen/C-2741-2009; Wang, Yu/C-1600-2010; Murtaza, Adil/K-7714-2016; Zhou, Chao/G-3661-2010 FU National Basic Research Program of China [2012CB619401]; National Natural Science Foundation of China [51222104, 51371134, 51471125, 51431007]; Program for Key Science and Technology Innovative Team of Shaanxi Province [2013KCT-05]; Collaborative Innovation Center of Suzhou Nano Science and Technology; U.S. Department of Energy [DE-AC02-06CH11357] FX This work was supported by the National Basic Research Program of China (Grant No. 2012CB619401), National Natural Science Foundation of China (Grant Nos. 51222104, 51371134, 51471125, and 51431007), Program for Key Science and Technology Innovative Team of Shaanxi Province (No. 2013KCT-05), and Collaborative Innovation Center of Suzhou Nano Science and Technology. Use of the Advanced Photon Source at Argonne National Laboratory was supported by the U.S. Department of Energy (DE-AC02-06CH11357). We thank Dr. Matthrew Suchomel for his great help with the high-resolution synchrotron x-ray diffraction experiment at 11-BM-B. NR 34 TC 6 Z9 6 U1 8 U2 52 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAR 30 PY 2015 VL 106 IS 13 AR 132403 DI 10.1063/1.4916652 PG 5 WC Physics, Applied SC Physics GA CF1MT UT WOS:000352310700029 ER PT J AU Cai, S Schaffer, JE Ren, Y AF Cai, S. Schaffer, J. E. Ren, Y. TI Deformation of a Ti-Nb alloy containing alpha ''-martensite and omega phases SO APPLIED PHYSICS LETTERS LA English DT Article ID TRANSMISSION ELECTRON-MICROSCOPY; MECHANICAL-PROPERTIES; GUM METAL; TRANSFORMATION; TEXTURE; EVOLUTION AB Microscopic deformation of a Ti-17at. %Nb alloy with high fractions of alpha"-martensite and omega phases was studied by in-situ synchrotron X-ray diffraction. Textures, phase fractions, individual lattice strains, and peak intensities during deformation were studied. It is found that, to accommodate the external tensile strain, some of the alpha" and omega grains were first transformed to the beta-phase, which then continuously transformed to the alpha"-phase with chosen variants that effectively accommodate the deformation strain. A strong (010)(alpha") fiber texture was formed at the expense of the (001)(alpha") and (111)(alpha") fiber textures. Above 400 MPa applied stress, (110)(alpha") deformation twinning was triggered with a simultaneous stress relaxation in the (110)(alpha") family and a slight increase in its texture strength in the loading direction. (C) 2015 AIP Publishing LLC. C1 [Cai, S.; Schaffer, J. E.] Ft Wayne Met Res Prod Corp, Ft Wayne, IN 46809 USA. [Ren, Y.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Cai, S (reprint author), Ft Wayne Met Res Prod Corp, 9609 Ardmore Ave, Ft Wayne, IN 46809 USA. FU Fort Wayne Metals Research Products Corporation; U.S. Department of Energy, Office of Science [DE-AC02-06CH11357] FX This study was funded by Fort Wayne Metals Research Products Corporation. Use of the synchrotron X-ray at APS was granted by the U.S. Department of Energy, Office of Science, under Contract No. DE-AC02-06CH11357. Data were analyzed by using the FIT2D, Maud, and GSAS software. S. Cai thanks his colleague Adam Griebel for reading the manuscript and Dr. D. H. Ping from National Institute for Materials Science of Japan for numerous discussions. NR 20 TC 3 Z9 4 U1 3 U2 29 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAR 30 PY 2015 VL 106 IS 13 AR 131907 DI 10.1063/1.4916960 PG 5 WC Physics, Applied SC Physics GA CF1MT UT WOS:000352310700021 ER PT J AU Herklotz, A Dorr, K Ward, TZ Eres, G Christen, HM Biegalski, MD AF Herklotz, A. Doerr, K. Ward, T. Z. Eres, G. Christen, H. M. Biegalski, M. D. TI Stoichiometry control of complex oxides by sequential pulsed-laser deposition from binary-oxide targets SO APPLIED PHYSICS LETTERS LA English DT Article ID MOLECULAR-BEAM EPITAXY; THIN-FILMS; GROWTH AB To have precise atomic layer control over interfaces, we examine the growth of complex oxides through the sequential deposition from binary targets by pulsed laser deposition. In situ reflection high-energy electron diffraction (RHEED) is used to control the growth and achieve films with excellent structural quality. The growth from binary oxide targets is fundamentally different from single target growth modes and shows more similarities to shuttered growth by molecular beam epitaxy. The RHEED intensity oscillations of non-stoichiometric growth are consistent with a model of island growth and accumulation of excess material on the surface that can be utilized to determine the correct stoichiometry for growth. Correct monolayer doses can be determined through an envelope frequency in the RHEED intensity oscillations. In order to demonstrate the ability of this growth technique to create complex heterostructures, the artificial n = 2 and 3 Srn+1TinO3n+1 Ruddlesden-Popper phases are grown with good long-range order. This method enables the precise unit-cell level control over the structure of perovskite-type oxides, and thus the growth of complex materials with improved structural quality and electronic functionality. (C) 2015 AIP Publishing LLC. C1 [Herklotz, A.; Ward, T. Z.; Eres, G.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Herklotz, A.; Doerr, K.] Univ Halle Wittenberg, Inst Phys, D-06120 Halle, Germany. [Christen, H. M.; Biegalski, M. D.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Herklotz, A (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Bethel Valley Rd, Oak Ridge, TN 37831 USA. RI Christen, Hans/H-6551-2013; Ward, Thomas/I-6636-2016; Eres, Gyula/C-4656-2017 OI Christen, Hans/0000-0001-8187-7469; Ward, Thomas/0000-0002-1027-9186; Eres, Gyula/0000-0003-2690-5214 FU DOE Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; [SFB 762] FX This research was conducted at the Center for Nanophase Materials Sciences, which is a U.S. Department of Energy (DOE), Office of Science User Facility. T.Z.W. and A.H. were supported by the DOE Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; A.H. and K.D. are grateful for the support by SFB 762. NR 26 TC 3 Z9 3 U1 3 U2 48 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAR 30 PY 2015 VL 106 IS 13 AR 131601 DI 10.1063/1.4916948 PG 4 WC Physics, Applied SC Physics GA CF1MT UT WOS:000352310700013 ER PT J AU Mahabaduge, HP Rance, WL Burst, JM Reese, MO Meysing, DM Wolden, CA Li, J Beach, JD Gessert, TA Metzger, WK Garner, S Barnes, TM AF Mahabaduge, H. P. Rance, W. L. Burst, J. M. Reese, M. O. Meysing, D. M. Wolden, C. A. Li, J. Beach, J. D. Gessert, T. A. Metzger, W. K. Garner, S. Barnes, T. M. TI High-efficiency, flexible CdTe solar cells on ultra-thin glass substrates SO APPLIED PHYSICS LETTERS LA English DT Article AB Flexible, high-efficiency, low-cost solar cells can enable applications that take advantage of high specific power, flexible form factors, lower installation and transportation costs. Here, we report a certified record efficiency of 16.4% for a flexible CdTe solar cell that is a marked improvement over the previous standard (14.05%). The improvement was achieved by replacing chemical-bath-deposited CdS with sputtered CdS:O and also replacing the high-temperature sputtered ZnTe:Cu back contact layer with co-evaporated and rapidly annealed ZnTe:Cu. We use quantum efficiency and capacitance-voltage measurements combined with device simulations to identify the reasons for the increase in efficiency. Both device simulations and experimental results show that higher carrier density can quantitatively account for the increased open circuit voltage (V-OC) and Fill Factor (FF), and likewise, the increase in short circuit current density (J(SC)) can be attributed to the more transparent CdS:O. (C) 2015 AIP Publishing LLC. C1 [Mahabaduge, H. P.; Rance, W. L.; Burst, J. M.; Reese, M. O.; Gessert, T. A.; Metzger, W. K.; Barnes, T. M.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Meysing, D. M.; Wolden, C. A.; Li, J.; Beach, J. D.] Colorado Sch Mines, Golden, CO 80401 USA. [Garner, S.] Corning Inc, Corning, NY 14831 USA. RP Mahabaduge, HP (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. FU U.S. Department of Energy through the SunShot Foundational Program to Advance Cell Efficiency (F-PACE) [DE-AC36-08-GO28308]; Bay Area Photovoltaic Consortium FX This work was supported by the U.S. Department of Energy through the SunShot Foundational Program to Advance Cell Efficiency (F-PACE) under Contract No. DE-AC36-08-GO28308. J. D. Beach and J. Li were supported by the Bay Area Photovoltaic Consortium. NR 14 TC 19 Z9 19 U1 9 U2 43 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAR 30 PY 2015 VL 106 IS 13 AR 133501 DI 10.1063/1.4916634 PG 4 WC Physics, Applied SC Physics GA CF1MT UT WOS:000352310700052 ER PT J AU Coman, C Chiriac, CM Robeson, MS Ionescu, C Dragos, N Barbu-Tudoran, L Andrei, AS Banciu, HL Sicora, C Podar, M AF Coman, Cristian Chiriac, Cecilia M. Robeson, Michael S. Ionescu, Corina Dragos, Nicolae Barbu-Tudoran, Lucian Andrei, Adrian-Stefan Banciu, Horia L. Sicora, Cosmin Podar, Mircea TI Structure, mineralogy, and microbial diversity of geothermal spring microbialites associated with a deep oil drilling in Romania SO FRONTIERS IN MICROBIOLOGY LA English DT Article DE hot springs; carbonate; biomineralization; amplicon sequencing; microbial diversity; oil drill ID MODERN MARINE STROMATOLITES; POLYMERIC SECRETIONS EPS; MAXIMUM-LIKELIHOOD; WESTERN-AUSTRALIA; SHARK BAY; OXIDIZING BACTERIUM; COMMUNITY STRUCTURE; THROMBOLITIC MATS; CUATRO CIENEGAS; GENE-SEQUENCES AB Modern mineral deposits play an important role in evolutionary studies by providing clues to the formation of ancient lithified microbial communities. Here we report the presence of microbialite-forming microbial mats in different microenvironments at 32 degrees C, 49 degrees C, and 65 degrees C around the geothermal spring from an abandoned oil drill in Ciocaia, Romania. The mineralogy and the macro- and microstructure of the microbialites were investigated, together with their microbial diversity based on a 16S rRNA gene amplicon sequencing approach. The calcium carbonate is deposited mainly in the form of calcite. At 32 degrees C and 49 degrees C, the microbialites show a laminated structure with visible microbial mat-carbonate crystal interactions. At 65 degrees C, the mineral deposit is clotted, without obvious organic residues. Partial 16S rRNA gene amplicon sequencing showed that the relative abundance of the phylum Archaea was low at 32 degrees C (<0.5%) but increased significantly at 65 degrees C (36%). The bacterial diversity was either similar to other microbialites described in literature (the 32 degrees C sample) or displayed a specific combination of phyla and classes (the 49 degrees C and 65 degrees C samples). Bacterial taxa were distributed among 39 phyla, out of which 14 had inferred abundances >1%. The dominant bacterial groups at 32 degrees C were Cyanobacteria, Gammaproteobacteria, Firmicutes, Bacteroidetes, Chloroflexi, Thermi, Actinobacteria, Planctomycetes, and Defferibacteres. At 49 degrees C, there was a striking dominance of the Gammaproteobacteria, followed by Firmicutes, Bacteroidetes, and Armantimonadetes. The 65 degrees C sample was dominated by Betaproteobacteria, Firmicutes, [OP1], Defferibacteres, Thermi, Thermotogae, [EM3], and Nitrospirae. Several groups from Proteobacteria and Firmicutes, together with Halobacteria and Melainabacteria were described for the first time in calcium carbonate deposits. Overall, the spring from Ciocaia emerges as a valuable site to probe microbes-minerals interrelationships along thermal and geochemical gradients. C1 [Coman, Cristian; Chiriac, Cecilia M.; Dragos, Nicolae] Inst Biol Res, Natl Inst Res & Dev Biol Sci, Taxon & Ecol, Algol, Cluj Napoca 400015, Romania. [Coman, Cristian; Chiriac, Cecilia M.; Dragos, Nicolae; Banciu, Horia L.] Univ Babes Bolyai, Fac Biol & Geol, Dept Mol Biol & Biotechnol, R-3400 Cluj Napoca, Romania. [Robeson, Michael S.; Podar, Mircea] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN USA. [Robeson, Michael S.] Colorado State Univ, Fish Wildlife & Conservat Biol, Ft Collins, CO 80523 USA. [Ionescu, Corina] Univ Babes Bolyai, Fac Biol & Geol, Dept Geol, R-3400 Cluj Napoca, Romania. [Ionescu, Corina] Kazan Volga Reg Fed Univ, Tatarstan, Russia. [Barbu-Tudoran, Lucian] Univ Babes Bolyai, Fac Biol & Geol, Ctr Electron Microscopy, R-3400 Cluj Napoca, Romania. [Andrei, Adrian-Stefan; Banciu, Horia L.] Univ Babes Bolyai, Ctr Mol Biol, Inst Interdisciplinary Res Bionanosci, R-3400 Cluj Napoca, Romania. [Sicora, Cosmin] Biol Res Ctr, Jibou, Romania. RP Coman, C (reprint author), Inst Biol Res, 48 Republ St, Cluj Napoca 400015, Romania. EM cristian.coman@icbcluj.ro RI IONESCU, CORINA/B-8868-2011; Banciu, Horia /B-7433-2011; OI IONESCU, CORINA/0000-0001-8704-9816; Banciu, Horia /0000-0002-6563-3226; Podar, Mircea/0000-0003-2776-0205; Robeson, Michael/0000-0001-7119-6301; Barbu-Tudoran, Lucian/0000-0003-0360-016X; Andrei, Adrian-Stefan/0000-0003-1425-7168 FU CNCS-UEFIS-CDI [PN-II-ID-PCE-2011-3-0546]; Russian Government; Oak Ridge National Laboratory (ORNL); [PD 104/2012]; [PN 09-360201]; [POSDRU/159/1.5/S/133391]; [POSDRU/159/1.5/S/132400] FX CC and CMC were supported by grants PD 104/2012 and PN 09-360201. CC was also supported by the strategic grant POSDRU/159/1.5/S/133391. AA-S and HLB were supported by CNCS-UEFIS-CDI, project number PN-II-ID-PCE-2011-3-0546. AA-S was also supported by a POSDRU/159/1.5/S/132400 research scholarship. CI acknowledges subsidy of the Russian Government to support the "Program of competitive growth of Kazan Federal University among world class academic centers and universities." MR and MP were supported by Oak Ridge National Laboratory (ORNL). ORNL is managed by UT-Battelle, LLC, for the U.S. Department of Energy. We thank Zamin Yang and Dawn Klingeman for help with Illumina amplicon preparation and sequencing. NR 105 TC 4 Z9 4 U1 6 U2 25 PU FRONTIERS RESEARCH FOUNDATION PI LAUSANNE PA PO BOX 110, LAUSANNE, 1015, SWITZERLAND SN 1664-302X J9 FRONT MICROBIOL JI Front. Microbiol. PD MAR 30 PY 2015 VL 6 AR 253 DI 10.3389/fmicb.2015.00253 PG 14 WC Microbiology SC Microbiology GA CF4QV UT WOS:000352536500001 PM 25870594 ER PT J AU Tsitoura, F Kruger, P Kevrekidis, PG Frantzeskakis, DJ AF Tsitoura, F. Krueger, P. Kevrekidis, P. G. Frantzeskakis, D. J. TI Scattering of matter waves in spatially inhomogeneous environments SO PHYSICAL REVIEW A LA English DT Article ID BOSE-EINSTEIN CONDENSATE; LIGHT-BEAM PROPAGATION; FESHBACH RESONANCES; NONLINEAR INTERFACES; DARK SOLITONS; ATOM OPTICS; COLLISIONS; DYNAMICS; PARTICLE; RB-85 AB We study scattering of quasi-one-dimensional matter waves at an interface of two spatial domains, one with repulsive and one with attractive interatomic interactions. It is shown that the incidence of a Gaussian wave packet from the repulsive to the attractive region gives rise to generation of a soliton train. More specifically, the number of emergent solitons can be controlled, e.g., by the variation of the amplitude or the width of the incoming wave packet. Furthermore, we study the reflectivity of a soliton incident from the attractive region to the repulsive one. We find the reflection coefficient numerically and employ analytical methods, which treat the soliton as a particle (for moderate and large amplitudes) or a quasilinear wave packet (for small amplitudes), to determine the critical soliton momentum (as a function of the soliton amplitude) for which total reflection is observed. C1 [Tsitoura, F.; Frantzeskakis, D. J.] Univ Athens, Dept Phys, Athens 15784, Greece. [Krueger, P.] Univ Nottingham, Sch Phys & Astron, Midlands Ultracold Atom Res Ctr, Nottingham NG7 1AX, England. [Kevrekidis, P. G.] Univ Massachusetts, Dept Math & Stat, Amherst, MA 01003 USA. [Kevrekidis, P. G.] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87544 USA. [Kevrekidis, P. G.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87544 USA. RP Tsitoura, F (reprint author), Univ Athens, Dept Phys, Athens 15784, Greece. OI Kruger, Peter/0000-0001-9908-6454 FU University of Athens; National Science Foundation [DMS-1312856]; FP7-People [IRSES-605096]; Binational (US-Israel) Science Foundation [2010239]; US AFOSR [FA9550-12-10332]; EPSRC [EP/I017828/1]; EU [FP7-ICT-601180, FP7-ICT-250072]; US Department of Energy FX The work of D.J.F. was partially supported by the Special Account for Research Grants of the University of Athens. P.G.K. acknowledges support from the National Science Foundation under Grant No. DMS-1312856, FP7-People under Grant No. IRSES-605096, the Binational (US-Israel) Science Foundation through Grant No. 2010239, and the US AFOSR under Grant No. FA9550-12-10332. P.K. acknowledges support from EPSRC (Grant No. EP/I017828/1) and the EU (Grants No. FP7-ICT-601180 and No. FP7-ICT-250072). P.G.K. and P.K. also acknowledge the hospitality of the Synthetic Quantum Systems group and of Markus Oberthaler at the Kirchhoff Institute for Physics at the University of Heidelberg, the Center for Optical Quantum Technologies and Peter Schmelcher at the University of Hamburg, and the Center for Nonlinear Studies at the Los Alamos National Laboratory. The work of P.G.K. at Los Alamos was supported in part by the US Department of Energy. NR 69 TC 2 Z9 2 U1 1 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9926 EI 2469-9934 J9 PHYS REV A JI Phys. Rev. A PD MAR 30 PY 2015 VL 91 IS 3 AR 033633 DI 10.1103/PhysRevA.91.033633 PG 8 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA CE9WZ UT WOS:000352195500016 ER PT J AU Agnese, R Anderson, AJ Balakishiyeva, D Thakur, RB Bauer, DA Billard, J Borgland, A Bowles, MA Brandt, D Brink, PL Bunker, R Cabrera, B Caldwell, DO Cerdeno, DG Chagani, H Chen, Y Cooley, J Cornell, B Crewdson, CH Cushman, P Daal, M Di Stefano, PCF Doughty, T Esteban, L Fallows, S Figueroa-Feliciano, E Fritts, M Godfrey, GL Golwala, SR Graham, M Hall, J Harris, HR Hertel, SA Hofer, T Holmgren, D Hsu, L Huber, ME Jastram, A Kamaev, O Kara, B Kelsey, MH Kennedy, A Kiveni, M Koch, K Leder, A Loer, B Asamar, EL Mahapatra, R Mandic, V Martinez, C McCarthy, KA Mirabolfathi, N Moffatt, RA Moore, DC Nelson, RH Oser, SM Page, K Page, WA Partridge, R Pepin, M Phipps, A Prasad, K Pyle, M Qiu, H Rau, W Redl, P Reisetter, A Ricci, Y Rogers, HE Saab, T Sadoulet, B Sander, J Schneck, K Schnee, RW Scorza, S Serfass, B Shank, B Speller, D Upadhyayula, S Villano, AN Welliver, B Wright, DH Yellin, S Yen, JJ Young, BA Zhang, J AF Agnese, R. Anderson, A. J. Balakishiyeva, D. Thakur, R. Basu Bauer, D. A. Billard, J. Borgland, A. Bowles, M. A. Brandt, D. Brink, P. L. Bunker, R. Cabrera, B. Caldwell, D. O. Cerdeno, D. G. Chagani, H. Chen, Y. Cooley, J. Cornell, B. Crewdson, C. H. Cushman, P. Daal, M. Di Stefano, P. C. F. Doughty, T. Esteban, L. Fallows, S. Figueroa-Feliciano, E. Fritts, M. Godfrey, G. L. Golwala, S. R. Graham, M. Hall, J. Harris, H. R. Hertel, S. A. Hofer, T. Holmgren, D. Hsu, L. Huber, M. E. Jastram, A. Kamaev, O. Kara, B. Kelsey, M. H. Kennedy, A. Kiveni, M. Koch, K. Leder, A. Loer, B. Lopez Asamar, E. Mahapatra, R. Mandic, V. Martinez, C. McCarthy, K. A. Mirabolfathi, N. Moffatt, R. A. Moore, D. C. Nelson, R. H. Oser, S. M. Page, K. Page, W. A. Partridge, R. Pepin, M. Phipps, A. Prasad, K. Pyle, M. Qiu, H. Rau, W. Redl, P. Reisetter, A. Ricci, Y. Rogers, H. E. Saab, T. Sadoulet, B. Sander, J. Schneck, K. Schnee, R. W. Scorza, S. Serfass, B. Shank, B. Speller, D. Upadhyayula, S. Villano, A. N. Welliver, B. Wright, D. H. Yellin, S. Yen, J. J. Young, B. A. Zhang, J. CA SuperCDMS Collaboration TI Maximum likelihood analysis of low energy CDMS II germanium data SO PHYSICAL REVIEW D LA English DT Article ID IONIZATION; DETECTORS; GEANT4 AB We report on the results of a search for a Weakly Interacting Massive Particle (WIMP) signal in low-energy data of the Cryogenic Dark Matter Search experiment using a maximum likelihood analysis. A background model is constructed using GEANT4 to simulate the surface-event background from Pb-210 decay-chain events, while using independent calibration data to model the gamma background. Fitting this background model to the data results in no statistically significant WIMP component. In addition, we perform fits using an analytic ad hoc background model proposed by Collar and Fields, who claimed to find a large excess of signal-like events in our data. We confirm the strong preference for a signal hypothesis in their analysis under these assumptions, but excesses are observed in both single-and multiple-scatter events, which implies the signal is not caused by WIMPs, but rather reflects the inadequacy of their background model. C1 [Cornell, B.; Golwala, S. R.; Moore, D. C.; Nelson, R. H.] CALTECH, Div Phys Math & Astron, Pasadena, CA 91125 USA. [Thakur, R. Basu; Bauer, D. A.; Holmgren, D.; Hsu, L.; Loer, B.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Sadoulet, B.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Anderson, A. J.; Billard, J.; Figueroa-Feliciano, E.; Hertel, S. A.; Leder, A.; McCarthy, K. A.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Hall, J.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Oser, S. M.; Page, W. A.] Univ British Columbia, Dept Phys & Astron, Vancouver, BC V6T 1Z1, Canada. [Crewdson, C. H.; Di Stefano, P. C. F.; Kamaev, O.; Martinez, C.; Page, K.; Rau, W.; Ricci, Y.] Queens Univ, Dept Phys, Kingston, ON K7L 3N6, Canada. [Young, B. A.] Santa Clara Univ, Dept Phys, Santa Clara, CA 95053 USA. [Borgland, A.; Brandt, D.; Brink, P. L.; Godfrey, G. L.; Graham, M.; Kelsey, M. H.; Partridge, R.; Schneck, K.; Wright, D. H.] SLAC Natl Accelerator Lab, Kavli Inst Particle Astrophys & Cosmol, Menlo Pk, CA 94025 USA. [Cooley, J.; Qiu, H.; Scorza, S.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Cabrera, B.; Moffatt, R. A.; Redl, P.; Shank, B.; Yellin, S.; Yen, J. J.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Bowles, M. A.; Bunker, R.; Chen, Y.; Kiveni, M.; Schnee, R. W.] Syracuse Univ, Dept Phys, Syracuse, NY 13244 USA. [Harris, H. R.; Jastram, A.; Mahapatra, R.; Mirabolfathi, N.; Prasad, K.; Upadhyayula, S.] Texas A&M Univ, Dept Phys, College Stn, TX 77843 USA. [Cerdeno, D. G.; Esteban, L.; Lopez Asamar, E.] Univ Autonoma Madrid, CSIC, Dept Fis Teor, E-28049 Madrid, Spain. [Cerdeno, D. G.; Esteban, L.; Lopez Asamar, E.] Univ Autonoma Madrid, CSIC, Inst Fis Teor, E-28049 Madrid, Spain. [Doughty, T.; Phipps, A.; Pyle, M.; Sadoulet, B.; Serfass, B.; Speller, D.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Caldwell, D. O.] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA. [Huber, M. E.] Univ Colorado, Dept Phys, Denver, CO 80217 USA. [Reisetter, A.] Univ Evansville, Dept Phys, Evansville, IN 47722 USA. [Agnese, R.; Balakishiyeva, D.; Saab, T.; Welliver, B.] Univ Florida, Dept Phys, Gainesville, FL 32611 USA. [Thakur, R. Basu] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Chagani, H.; Cushman, P.; Fallows, S.; Fritts, M.; Hofer, T.; Kennedy, A.; Koch, K.; Mandic, V.; Pepin, M.; Rogers, H. E.; Villano, A. N.; Zhang, J.] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Sander, J.] Univ S Dakota, Dept Phys, Vermillion, SD 57069 USA. RP Agnese, R (reprint author), Univ Florida, Dept Phys, Gainesville, FL 32611 USA. EM redl@stanford.edu RI Hall, Jeter/E-9294-2015; Pyle, Matt/E-7348-2015; OI Pyle, Matt/0000-0002-3490-6754; Cerdeno, David G./0000-0002-7649-1956 FU National Science Foundation; United States Department of Energy; NSERC Canada; MultiDark (Spanish MINECO); Fermi Research Alliance, LLC [De-AC02-07CH11359]; United States Department of Energy [DE-AC02-76SF00515] FX The CDMS Collaboration gratefully acknowledges the contributions of numerous engineers and technicians; we would like to especially thank Dennis Seitz, Jim Beaty, Bruce Hines, Larry Novak, Richard Schmitt, Astrid Tomada, and John Emes. In addition, we gratefully acknowledge assistance from the staff of the Soudan Underground Laboratory and the Minnesota Department of Natural Resources. This work is supported in part by the National Science Foundation, by the United States Department of Energy, by NSERC Canada, and by MultiDark (Spanish MINECO). Fermilab is operated by the Fermi Research Alliance, LLC under Contract No. De-AC02-07CH11359. SLAC is operated under Contract No. DE-AC02-76SF00515 with the United States Department of Energy. NR 26 TC 5 Z9 5 U1 6 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD MAR 30 PY 2015 VL 91 IS 5 AR 052021 DI 10.1103/PhysRevD.91.052021 PG 13 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CE9XP UT WOS:000352197200001 ER PT J AU Shi, X Pan, W Baldwin, KW West, KW Pfeiffer, LN Tsui, DC AF Shi, X. Pan, W. Baldwin, K. W. West, K. W. Pfeiffer, L. N. Tsui, D. C. TI Impact of the modulation doping layer on the nu=5/2 anisotropy SO PHYSICAL REVIEW B LA English DT Article ID HIGH LANDAU-LEVELS; INCOMPRESSIBLE QUANTUM FLUID; LEVEL FILLING FACTOR; MAGNETIC-FIELD; HALL STRIPES; STATES; LIQUID; QUANTIZATION; MECHANISMS; ELECTRONS AB We have carried out a systematic study of the tilted magnetic field induced anisotropy at the Landau level filling factor nu = 5/2 in a series of high quality GaAs quantum wells, where the setback distance (d) between the modulation doping layer and the GaAs quantum well is varied from 33 to 164 nm. We have observed that in the sample of the smallest d, electronic transport is anisotropic when the in-plane magnetic field (B-ip) is parallel to the [1-10] crystallographic direction, but remains more or less isotropic when B-ip parallel to [110]. In contrast, in the sample of largest d, electronic transport is anisotropic in both crystallographic directions. Our results clearly show that the modulation doping layer plays an important role in the tilted field induced nu = 5/2 anisotropy. C1 [Shi, X.; Pan, W.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Baldwin, K. W.; West, K. W.; Pfeiffer, L. N.; Tsui, D. C.] Princeton Univ, Princeton, NJ 08544 USA. RP Shi, X (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. RI Shi, Xiaoyan/L-4893-2015 OI Shi, Xiaoyan/0000-0002-9974-4637 FU Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; Gordon and Betty Moore Foundation; Keck Foundation; National Science Foundation MRSEC Program through Princeton Center for Complex Materials; National Science Foundation [DMR-1157490]; State of Florida; DOE FX We thank Michael Manfra for helpful discussions. This work was supported by the Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. Sample growth at Princeton University was partially funded by the Gordon and Betty Moore Foundation, Keck Foundation, as well as the National Science Foundation MRSEC Program through the Princeton Center for Complex Materials. A portion of the work was performed at the National High Magnetic Field Laboratory, which is supported by the National Science Foundation (Grant No. DMR-1157490), the State of Florida, and the DOE. We thank Tim Murphy, Ju-Hyun Park, and Glover Jones for experimental help. NR 44 TC 3 Z9 3 U1 1 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAR 30 PY 2015 VL 91 IS 12 AR 125308 DI 10.1103/PhysRevB.91.125308 PG 6 WC Physics, Condensed Matter SC Physics GA CE9XL UT WOS:000352196700008 ER PT J AU Taylor, AE Morrow, R Singh, DJ Calder, S Lumsden, MD Woodward, PM Christianson, AD AF Taylor, A. E. Morrow, R. Singh, D. J. Calder, S. Lumsden, M. D. Woodward, P. M. Christianson, A. D. TI Magnetic order and electronic structure of the 5d(3) double perovskite Sr2ScOsO6 SO PHYSICAL REVIEW B LA English DT Article ID NEUTRON-DIFFRACTION; CRYSTAL AB The magnetic susceptibility, crystal and magnetic structures, and electronic structure of the double perovskite Sr2ScOsO6 are reported. Using both neutron and x-ray powder diffraction we find that the crystal structure is monoclinic P2(1)/n from 3.5 to 300 K. Magnetization measurements indicate an antiferromagnetic transition at T-N = 92 K, one of the highest transition temperatures of any double perovskite hosting only one magnetic ion. Type I antiferromagnetic order is determined by neutron powder diffraction, with an Os moment of only 1.6(1)mu(B), close to half the spin-only value for a crystal field split 5d electron state with a t(2g)(3) ground state. Density functional calculations show that this reduction is largely the result of strong Os-O hybridization, with spin-orbit coupling responsible for only a similar to 0.1 mu(B) reduction in the moment. C1 [Taylor, A. E.; Calder, S.; Lumsden, M. D.; Christianson, A. D.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Morrow, R.; Woodward, P. M.] Ohio State Univ, Dept Chem, Columbus, OH 43210 USA. [Singh, D. J.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Christianson, A. D.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. RP Taylor, AE (reprint author), Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. EM taylorae@ornl.gov RI Taylor, Alice/I-5616-2012; Morrow, Ryan/K-9668-2015; christianson, andrew/A-3277-2016; Lumsden, Mark/F-5366-2012 OI Taylor, Alice/0000-0002-3036-3019; Morrow, Ryan/0000-0001-9986-3049; christianson, andrew/0000-0003-3369-5884; Lumsden, Mark/0000-0002-5472-9660 FU Center for Emergent Materials an NSF Materials Research Science and Engineering Center [DMR-0820414]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy (DOE); U.S. Department of Energy [DE-AC05-00OR22725] FX Support for this research was provided by the Center for Emergent Materials an NSF Materials Research Science and Engineering Center (DMR-0820414). The research at ORNL's Spallation Neutron Source and High Flux Isotope Reactor was supported by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy (DOE). The theoretical calculations (D.J.S.) were supported by the Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. The authors gratefully acknowledge A. Huq for providing help with the experimental work on POWGEN, and J.Q. Yan, D. Mandrus, and B. Sales for useful discussions. This manuscript has been authored by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The U.S. Government retains a nonexclusive, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for U.S. Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan. NR 41 TC 18 Z9 18 U1 8 U2 42 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAR 30 PY 2015 VL 91 IS 10 AR 100406 DI 10.1103/PhysRevB.91.100406 PG 5 WC Physics, Condensed Matter SC Physics GA CE9XH UT WOS:000352196300002 ER PT J AU Yamaoka, H Schwier, EF Arita, M Shimada, K Tsujii, N Jarrige, I Jiang, J Hayashi, H Iwasawa, H Namatame, H Taniguchi, M Kitazawa, H AF Yamaoka, Hitoshi Schwier, Eike F. Arita, Masashi Shimada, Kenya Tsujii, Naohito Jarrige, Ignace Jiang, Jian Hayashi, Hirokazu Iwasawa, Hideaki Namatame, Hirofumi Taniguchi, Masaki Kitazawa, Hideaki TI Electronic structure of the heavy-fermion caged compound Ce3Pd20X6 (X = Si, Ge) studied by density functional theory and photoelectron spectroscopy SO PHYSICAL REVIEW B LA English DT Article ID TEMPERATURE PHOTOEMISSION SPECTROSCOPY; HIGH-RESOLUTION; UNDULATOR BEAMLINE; KONDO SYSTEM; PRESSURE; LA AB The electronic structure of Ce3Pd20X6 (X = Si, Ge) has been studied using detailed density functional theory (DFT) calculations and high-resolution photoelectron spectroscopy (PES) measurements. The orbital decomposition of the electronic structure by DFT calculations indicates that Ce atoms at the (8c) site surrounded by 16 Pd atoms have a tendency to be magnetic. Ce atoms at the (4a) site surrounded by 12 Pd and 6 X atoms, on the other hand, are more localized and paramagnetic. The 4d-4f resonance PES measurements clearly indicate the Ce 4f contribution in the valence band in these compounds. The spectral weight of Ce 4f(0) is stronger than that of Ce 4f(1), indicating the localized nature of Ce 4f electrons. Near the Fermi level, the Ce 4f(1) weight of Ce3Pd20Si6 is stronger than that of Ce3Pd20Ge6, suggesting stronger c-f hybridization in the former. C1 [Yamaoka, Hitoshi] RIKEN, RIKEN SPring Ctr 8, Sayo, Hyogo 6795148, Japan. [Schwier, Eike F.; Arita, Masashi; Shimada, Kenya; Iwasawa, Hideaki; Namatame, Hirofumi; Taniguchi, Masaki] Hiroshima Univ, Hiroshima Synchrotron Radiat Ctr, Hiroshima 7390046, Japan. [Tsujii, Naohito; Kitazawa, Hideaki] Natl Inst Mat Sci, Quantum Beam Ctr, Tsukuba, Ibaraki 3050047, Japan. [Jarrige, Ignace] Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA. [Jiang, Jian; Hayashi, Hirokazu; Namatame, Hirofumi; Taniguchi, Masaki] Hiroshima Univ, Grad Sch Sci, Hiroshima 7390046, Japan. RP Yamaoka, H (reprint author), RIKEN, RIKEN SPring Ctr 8, 1-1-1 Kouto, Sayo, Hyogo 6795148, Japan. EM yamaoka@spring8.or.jp; schwier@hiroshima-u.ac.jp RI Shimada, Kenya/G-5080-2016; Jarrige, Ignace/M-6371-2016; Tsujii, Naohito/H-2544-2011; OI Shimada, Kenya/0000-0002-1945-2352; Jarrige, Ignace/0000-0002-1043-5695; Tsujii, Naohito/0000-0002-6181-5911; Schwier, Eike/0000-0003-3881-4045 FU JSPS; Alexander von Humboldt Foundation [P13783]; Swiss National Foundation [PBFRP2_140028] FX The experiments were performed at HiSOR beamlines BL-1 and BL-9A (HiSOR under Proposal Nos. 11-A-10 and 12-A-1) at Hiroshima University. We thank the N-BARD, Hiroshima University, for supplying the liquid helium as well as P. Aebi for helpful discussion. E.F.S acknowledges financial support from the JSPS postdoctoral fellowship for overseas researchers as well as the Alexander von Humboldt Foundation (Grant No. P13783) and the Swiss National Foundation fellowship for prospective researchers (Grant No. PBFRP2_140028). NR 43 TC 2 Z9 2 U1 8 U2 19 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 30 PY 2015 VL 91 IS 11 AR 115139 DI 10.1103/PhysRevB.91.115139 PG 9 WC Physics, Condensed Matter SC Physics GA CE9XJ UT WOS:000352196500001 ER PT J AU Nakata, H Fedorov, DG Zahariev, F Schmidt, MW Kitaura, K Gordon, MS Nakamura, S AF Nakata, Hiroya Fedorov, Dmitri G. Zahariev, Federico Schmidt, Michael W. Kitaura, Kazuo Gordon, Mark S. Nakamura, Shinichiro TI Analytic second derivative of the energy for density functional theory based on the three-body fragment molecular orbital method SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID HARMONIC VIBRATIONAL FREQUENCIES; HARTREE-FOCK CALCULATIONS; 2ND DERIVATIVES; WEIGHT DERIVATIVES; LARGE SYSTEMS; CONFIGURATION-INTERACTION; ACCURATE CALCULATIONS; DYNAMICS SIMULATIONS; POLYATOMIC-MOLECULES; FORCE CONSTANTS AB Analytic second derivatives of the energy with respect to nuclear coordinates have been developed for spin restricted density functional theory (DFT) based on the fragment molecular orbital method (FMO). The derivations were carried out for the three-body expansion (FMO3), and the two-body expressions can be obtained by neglecting the three-body corrections. Also, the restricted Hartree-Fock (RHF) Hessian for FMO3 can be obtained by neglecting the density-functional related terms. In both the FMO-RHF and FMO-DFT Hessians, certain terms with small magnitudes are neglected for computational efficiency. The accuracy of the FMO-DFT Hessian in terms of the Gibbs free energy is evaluated for a set of polypeptides and water clusters and found to be within 1 kcal/mol of the corresponding full (non-fragmented) ab initio calculation. The FMO-DFT method is also applied to transition states in S(N)2 reactions and for the computation of the IR and Raman spectra of a small Trp-cage protein (PDB: 1L2Y). Some computational timing analysis is also presented. (C) 2015 AIP Publishing LLC. C1 [Nakata, Hiroya] Tokyo Inst Technol, Ctr Biol Resources & Informat, Midori Ku, Yokohama, Kanagawa 2268501, Japan. [Nakata, Hiroya; Nakamura, Shinichiro] RIKEN, Res Cluster Innovat, Nakamura Lab, Wako, Saitama 3510198, Japan. [Nakata, Hiroya] Japan Soc Promot Sci, Chiyoda Ku, Tokyo 1020083, Japan. [Fedorov, Dmitri G.] Natl Inst Adv Ind Sci & Technol, NRI, Tsukuba, Ibaraki 3058568, Japan. [Zahariev, Federico; Schmidt, Michael W.; Gordon, Mark S.] Iowa State Univ, US DOE, Dept Chem, Ames, IA 50011 USA. [Zahariev, Federico; Schmidt, Michael W.; Gordon, Mark S.] Iowa State Univ, US DOE, Ames Lab, Ames, IA 50011 USA. [Kitaura, Kazuo] Kobe Univ, Grad Sch Syst Informat, Nada Ku, Kobe, Hyogo 6578501, Japan. RP Nakata, H (reprint author), Tokyo Inst Technol, Ctr Biol Resources & Informat, Midori Ku, B 62 4259 Nagatsuta Cho, Yokohama, Kanagawa 2268501, Japan. EM nakata.h.ab@m.titech.ac.jp; d.g.fedorov@aist.go.jp FU Next Generation Super Computing Project, Nanoscience Program (MEXT, Japan); Computational Materials Science Initiative (CMSI, Japan); JSPS KAKENHI [262235]; Department of Energy, Basic Energy Sciences; U.S. Department of Energy [DE-AC02-07CH11358] FX This work was in part supported by the Next Generation Super Computing Project, Nanoscience Program (MEXT, Japan) and Computational Materials Science Initiative (CMSI, Japan), and JSPS KAKENHI Grant No. 262235. H.N. acknowledges the use of the following computer resources: TSUBAME2.5 at the Global Scientific Information and Computing Center of Tokyo Institute of Technology, RIKEN Integrated Cluster of Clusters (RICC) at RIKEN. M.W.S., F.Z., and M.S.G. were supported by funds provided by the Department of Energy, Basic Energy Sciences, to the Ames Laboratory, administered by Iowa State University. The Ames Laboratory is operated for the U.S. Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. NR 96 TC 2 Z9 2 U1 0 U2 18 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAR 28 PY 2015 VL 142 IS 12 AR 124101 DI 10.1063/1.4915068 PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CF1OS UT WOS:000352316700003 ER PT J AU Newman, BD Throckmorton, HM Graham, DE Gu, B Hubbard, SS Liang, L Wu, Y Heikoop, JM Herndon, EM Phelps, TJ Wilson, CJ Wullschleger, SD AF Newman, B. D. Throckmorton, H. M. Graham, D. E. Gu, B. Hubbard, S. S. Liang, L. Wu, Y. Heikoop, J. M. Herndon, E. M. Phelps, T. J. Wilson, C. J. Wullschleger, S. D. TI Microtopographic and depth controls on active layer chemistry in Arctic polygonal ground SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE Arctic; permafrost; polygonal ground; active layer; geochemistry ID THAW-LAKE BASINS; NEAR-SURFACE PERMAFROST; COASTAL-PLAIN; TUNDRA ECOSYSTEMS; NORTHWEST-TERRITORIES; CARBON BALANCE; ALASKA; CANADA; ENVIRONMENT; FERTILIZATION AB Polygonal ground is a signature characteristic of Arctic lowlands, and carbon release from permafrost thaw can alter feedbacks to Arctic ecosystems and climate. This study describes the first comprehensive spatial examination of active layer biogeochemistry that extends across high- and low-centered, ice wedge polygons, their features, and with depth. Water chemistry measurements of 54 analytes were made on surface and active layer pore waters collected near Barrow, Alaska, USA. Significant differences were observed between high- and low-centered polygons suggesting that polygon types may be useful for landscape-scale geochemical classification. However, differences were found for polygon features (centers and troughs) for analytes that were not significant for polygon type, suggesting that finer-scale features affect biogeochemistry differently from polygon types. Depth variations were also significant, demonstrating important multidimensional aspects of polygonal ground biogeochemistry. These results have major implications for understanding how polygonal ground ecosystems function, and how they may respond to future change. C1 [Newman, B. D.; Throckmorton, H. M.; Heikoop, J. M.; Wilson, C. J.] Los Alamos Natl Lab, Div Earth & Environm Sci, Los Alamos, NM 87545 USA. [Graham, D. E.; Herndon, E. M.; Phelps, T. J.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN USA. [Gu, B.; Liang, L.; Wullschleger, S. D.] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. [Hubbard, S. S.; Wu, Y.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Newman, BD (reprint author), Los Alamos Natl Lab, Div Earth & Environm Sci, Los Alamos, NM 87545 USA. EM bnewman@lanl.gov RI Wu, Yuxin/G-1630-2012; Liang, Liyuan/O-7213-2014; Graham, David/F-8578-2010; Heikoop, Jeffrey/C-1163-2011; Hubbard, Susan/E-9508-2010; Gu, Baohua/B-9511-2012; Wullschleger, Stan/B-8297-2012 OI Wu, Yuxin/0000-0002-6953-0179; Liang, Liyuan/0000-0003-1338-0324; Heikoop, Jeffrey/0000-0001-7648-3385; Graham, David/0000-0001-8968-7344; Gu, Baohua/0000-0002-7299-2956; Wullschleger, Stan/0000-0002-9869-0446 FU Office of Biological and Environmental Research in the DOE Office of Science FX The Next-Generation Ecosystem Experiments (NGEE-Arctic) project is supported by the Office of Biological and Environmental Research in the DOE Office of Science. Review comments from John Gamon and an anonymous reviewer were much appreciated. We would also like to acknowledge Lily Cohen, Marvin Gard, Emily Kluk, Mike Rearick, George Perkins, and Xiangping Yin for their technical assistance and UMIAQ, LLC for logistical support in Barrow. Data used in this study can be obtained by contacting the corresponding author. NR 52 TC 6 Z9 6 U1 3 U2 20 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD MAR 28 PY 2015 VL 42 IS 6 BP 1808 EP 1817 DI 10.1002/2014GL062804 PG 10 WC Geosciences, Multidisciplinary SC Geology GA CG3HJ UT WOS:000353170000025 ER PT J AU Yu, HB Chin, M Yuan, TL Bian, HS Remer, LA Prospero, JM Omar, A Winker, D Yang, YK Zhang, Y Zhang, ZB Zhao, C AF Yu, Hongbin Chin, Mian Yuan, Tianle Bian, Huisheng Remer, Lorraine A. Prospero, Joseph M. Omar, Ali Winker, David Yang, Yuekui Zhang, Yan Zhang, Zhibo Zhao, Chun TI The fertilizing role of African dust in the Amazon rainforest: A first multiyear assessment based on data from Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE dust deposition; phosphorus; biogeochemical cycle; CALIPSO; satellite remote sensing; Amazon rainforest ID CLIMATE-CHANGE; SAHARAN DUST; TRANSPORT; BASIN; DEFORESTATION; PERSPECTIVE; AMERICA; CALIOP; MODEL; WET AB The productivity of the Amazon rainforest is constrained by the availability of nutrients, in particular phosphorus (P). Deposition of long-range transported African dust is recognized as a potentially important but poorly quantified source of phosphorus. This study provides a first multiyear satellite-based estimate of dust deposition into the Amazon Basin using three-dimensional (3-D) aerosol measurements over 2007-2013 from the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP). The 7year average of dust deposition into the Amazon Basin is estimated to be 28 (8-48)Tga(-1) or 29 (8-50)kgha(-1)a(-1). The dust deposition shows significant interannual variation that is negatively correlated with the prior-year rainfall in the Sahel. The CALIOP-based multiyear mean estimate of dust deposition matches better with estimates from in situ measurements and model simulations than a previous satellite-based estimate does. The closer agreement benefits from a more realistic geographic definition of the Amazon Basin and inclusion of meridional dust transport calculation in addition to the 3-D nature of CALIOP aerosol measurements. The imported dust could provide about 0.022(0.006-0.037)TgP of phosphorus per year, equivalent to 23 (7-39)gPha(-1)a(-1) to fertilize the Amazon rainforest. This out-of-basin phosphorus input is comparable to the hydrological loss of phosphorus from the basin, suggesting an important role of African dust in preventing phosphorus depletion on timescales of decades to centuries. C1 [Yu, Hongbin] Univ Maryland, Earth Syst Sci Interdisciplinary Ctr, College Pk, MD 20742 USA. [Yu, Hongbin; Chin, Mian; Yuan, Tianle; Bian, Huisheng; Yang, Yuekui; Zhang, Yan] NASA, Goddard Space Flight Ctr, Div Earth Sci, Greenbelt, MD 20771 USA. [Yuan, Tianle; Bian, Huisheng; Remer, Lorraine A.] Univ Maryland Baltimore Cty, Joint Ctr Earth Sci & Technol, Baltimore, MD 21228 USA. [Prospero, Joseph M.] Univ Miami, Rosenstiel Sch Marine & Atmospher Sci, Cooperat Inst Marine & Atmospher Studies, Miami, FL 33149 USA. [Omar, Ali; Winker, David] NASA, Langley Res Ctr, Hampton, VA 23665 USA. [Yang, Yuekui; Zhang, Yan] Univ Space Res Assoc, Columbia, MD USA. [Zhang, Zhibo] Univ Maryland Baltimore Cty, Dept Phys, Baltimore, MD 21228 USA. [Zhao, Chun] Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. RP Yu, HB (reprint author), Univ Maryland, Earth Syst Sci Interdisciplinary Ctr, College Pk, MD 20742 USA. EM Hongbin.Yu@nasa.gov RI Yu, Hongbin/C-6485-2008; Zhang, Zhibo/D-1710-2010; Yuan, Tianle/D-3323-2011; Zhao, Chun/A-2581-2012; Yang, Yuekui/B-4326-2015; Chin, Mian/J-8354-2012; Omar, Ali/D-7102-2017; OI Yu, Hongbin/0000-0003-4706-1575; Zhang, Zhibo/0000-0001-9491-1654; Zhao, Chun/0000-0003-4693-7213; Omar, Ali/0000-0003-1871-9235; Prospero, Joseph/0000-0003-3608-6160 FU NASA CALIPSO/CloudSat project [NNX14AB21G]; Science of Terra and Aqua project [NNX11AH66G]; U.S. DOE as part of the Regional and Global Climate Modeling program; DOE [DE-AC05-76RL01830] FX The work was supported by NASA CALIPSO/CloudSat project (NNX14AB21G) managed by David Considine and the Science of Terra and Aqua project (NNX11AH66G) managed by Richard Eckman. Chun Zhao acknowledges the support by the U.S. DOE as part of the Regional and Global Climate Modeling program. The Pacific Northwest National Laboratory is operated for DOE by Battelle Memorial Institute under contract DE-AC05-76RL01830. We thank Kelly Elkins of NASA GSFC Science Visualization Studio for helping in laying out Figure 1. We are grateful to Paulo Artaxo for helpful discussion and Francois-Xavier Collard for sharing the PM10 measurements at Cayenne with us. We thank two anonymous reviewers for their helpful suggestions. The CALIPSO data were obtained from the NASA Langley Research Center Atmospheric Sciences Data Center. The SPI data were downloaded from http://jisao.washington.edu/data/sahel/ (doi: 10.6059/H5MW2F2Q). The GPCP version 2.2 rainfall data were downloaded from the Giovanni online data system, developed and maintained by the NASA GES DISC. The processed CALIPSO aerosol profiles, GEOS-5 wind profiles, and GOCART and WRF-Chem dust simulations are archived in NASA GSFC clusters and personal computers, which will be made available to readers per request to the corresponding author H.Y. at Hongbin.Yu@nasa.gov. NR 40 TC 25 Z9 25 U1 7 U2 50 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD MAR 28 PY 2015 VL 42 IS 6 BP 1984 EP 1991 DI 10.1002/2015GL063040 PG 8 WC Geosciences, Multidisciplinary SC Geology GA CG3HJ UT WOS:000353170000047 ER PT J AU Carmer, J Jain, A Bollinger, JA van Swol, F Truskett, TM AF Carmer, James Jain, Avni Bollinger, Jonathan A. van Swol, Frank Truskett, Thomas M. TI Tuning structure and mobility of solvation shells surrounding tracer additives SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID UNIVERSAL SCALING LAW; POLYMER NANOCOMPOSITES; CONDENSED MATTER; CONFINED FLUIDS; EXCESS-ENTROPY; DIFFUSIVITY; LIQUIDS; COEFFICIENTS; PARTICLES; TRANSPORT AB Molecular dynamics simulations and a stochastic Fokker-Planck equation based approach are used to illuminate how position-dependent solvent mobility near one or more tracer particle(s) is affected when tracer-solvent interactions are rationally modified to affect corresponding solvation structure. For tracers in a dense hard-sphere fluid, we compare two types of tracer-solvent interactions: (1) a hard-sphere-like interaction, and (2) a soft repulsion extending beyond the hard core designed via statistical mechanical theory to enhance tracer mobility at infinite dilution by suppressing coordination-shell structure [Carmer et al., Soft Matter 8, 4083-4089 (2012)]. For the latter case, we show that the mobility of surrounding solvent particles is also increased by addition of the soft repulsive interaction, which helps to rationalize the mechanism underlying the tracer's enhanced diffusivity. However, if multiple tracer surfaces are in closer proximity (as at higher tracer concentrations), similar interactions that disrupt local solvation structure instead suppress the position-dependent solvent dynamics. (c) 2015 AIP Publishing LLC. C1 [Carmer, James; Jain, Avni; Bollinger, Jonathan A.; Truskett, Thomas M.] Univ Texas Austin, McKetta Dept Chem Engn, Austin, TX 78712 USA. [van Swol, Frank] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Carmer, J (reprint author), Univ Texas Austin, McKetta Dept Chem Engn, Austin, TX 78712 USA. EM truskett@che.utexas.edu RI Truskett, Thomas/D-4624-2009 OI Truskett, Thomas/0000-0002-6607-6468 FU Gulf of Mexico Research Initiative; Robert A. Welch Foundation [F-1696]; National Science Foundation [CBET-1403768]; United States Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; Sandia's LDRD program; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported by the Gulf of Mexico Research Initiative, the Robert A. Welch Foundation (F-1696) and the National Science Foundation (CBET-1403768). F.V.S. acknowledges support by the United States Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, and Sandia's LDRD program. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. We also acknowledge the Texas Advanced Computing Center (TACC) at The University of Texas at Austin for providing HPC resources for this study. NR 44 TC 4 Z9 4 U1 0 U2 9 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAR 28 PY 2015 VL 142 IS 12 AR 124501 DI 10.1063/1.4916053 PG 6 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CF1OS UT WOS:000352316700034 PM 25833590 ER PT J AU Fu, GS Zuo, L Chen, J Lu, M Yu, LY AF Fu, Gaosheng Zuo, Lei Chen, Jie Lu, Ming Yu, Liangyao TI Thermoelectric properties of DC-sputtered filled skutterudite thin film SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID PULSED-LASER DEPOSITION; THERMAL-CONDUCTIVITY; ENERGY-CONVERSION; P-TYPE; DEVICES; MERIT; POWER; FIGURE AB The Yb filled CoSb3 skutterudite thermoelectric thin films were prepared by DC magnetron sputtering. The electrical conductivity, Seebeck coefficient, thermal conductivity, and figure of merit ZT of the samples are characterized in a temperature range of 300K to 700 K. X-ray diffraction, scanning electron microscopy, and energy-dispersive X-ray spectroscopy are obtained to assess the phase composition and crystallinity of thin film samples at different heat treatment temperatures. Carrier concentrations and Hall mobilities are obtained from Hall Effect measurements, which provide further insight into the electrical conductivity and Seebeck coefficient mechanisms. The thermal conductivity of thin film filled skutterudite was found to be much less compared with bulk Yb filled CoSb3 skutterudite. In this work, the 1020K heat treatment was adopted for thin film post process due to the high degree of crystallinity as well as avoiding reverse heating effect. Thin film samples of different thicknesses were prepared with the same sputtering deposition rate and maximum ZT of 0.48 was achieved at 700K for the 130 nm thick sample. This value was between half and one third of the bulk figure of merit which was due to the lower Hall mobility. (C) 2015 AIP Publishing LLC. C1 [Fu, Gaosheng; Zuo, Lei] SUNY Stony Brook, Dept Mech Engn, Stony Brook, NY 11794 USA. [Zuo, Lei; Chen, Jie] Virginia Tech, Dept Mech Engn, Blacksburg, VA 24061 USA. [Lu, Ming] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Yu, Liangyao] Tsinghua Univ, State Key Lab Automot Safety & Energy, Beijing 10084, Peoples R China. RP Zuo, L (reprint author), SUNY Stony Brook, Dept Mech Engn, Stony Brook, NY 11794 USA. EM leizuo@vt.edu RI Zuo, Lei/B-3122-2017 FU NSF/DOE Thermoelectrics Partnership program under grant NSF CBET [1048744]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX The authors gratefully acknowledge financial support from the NSF/DOE Thermoelectrics Partnership program under grant NSF CBET #1048744. Research carried out in part at the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. The authors wish to thank Dr. Xiaoya Shi and Dr. Fernando Camino of Brookhaven National Laboratory and Mr. Shuyu Wang and Mr. Shifeng Yu of Stony Brook University for help in fabrication and characterization of the samples. Special thanks go to Dr. Richard Gambino for the insightful discussions and James Kierstead for the manuscript improvements. NR 34 TC 0 Z9 0 U1 1 U2 24 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAR 28 PY 2015 VL 117 IS 12 AR 125304 DI 10.1063/1.4916238 PG 7 WC Physics, Applied SC Physics GA CF1OJ UT WOS:000352315700051 ER PT J AU Xue, DZ Gao, JH Zhou, YM Ding, XD Sun, J Lookman, T Ren, XB AF Xue, Dezhen Gao, Jinghui Zhou, Yumei Ding, Xiangdong Sun, Jun Lookman, Turab Ren, Xiaobing TI Phase transitions and phase diagram of Ba(Zr0.2Ti0.8)O-3-x(Ba0.7Ca0.3)TiO3 Pb-free system by anelastic measurement SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID LEAD-FREE PIEZOCERAMICS; PIEZOELECTRIC CERAMICS; BOUNDARIES; COEXISTENCE; BEHAVIOR; MOTION; ORIGIN; PZT AB The internal friction and storage modulus of Ba(Zr0.2Ti0.8)O-3-x(Ba0.7Ca0.3)TiO3 (BZT-xBCT) Pb-free ceramics have been measured by dynamic mechanical analysis. The anelastic properties show clear anomalies with regard to the transformations between cubic (C), tetragonal (T), orthorhombic (O), and rhombohedral (R) phases, which are all of ferroelastic in nature. The previous reported T-R transition region in the BZT-xBCT system can be divided into the T-O and O-R transitions, consistent with recent studies on the appearance of an intermediate O phase. Based on the internal friction and storage modulus results, a revisited version of BZT-xBCT phase diagram is proposed. (C) 2015 AIP Publishing LLC. C1 [Xue, Dezhen; Gao, Jinghui; Zhou, Yumei; Ding, Xiangdong; Sun, Jun; Ren, Xiaobing] Xi An Jiao Tong Univ, Frontier Inst Sci & Technol, Multidisciplinary Mat Res Ctr, State Key Lab Mech Behav Mat, Xian 710049, Peoples R China. [Xue, Dezhen; Lookman, Turab] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Gao, Jinghui] Xi An Jiao Tong Univ, State Key Lab Elect Insulat & Power Equipment, Xian 710049, Peoples R China. [Ren, Xiaobing] Natl Inst Mat Sci, Ferro Phys Grp, Tsukuba, Ibaraki 3050047, Japan. RP Xue, DZ (reprint author), Xi An Jiao Tong Univ, Frontier Inst Sci & Technol, Multidisciplinary Mat Res Ctr, State Key Lab Mech Behav Mat, Xian 710049, Peoples R China. EM zhouyumei@mail.xjtu.edu.cn RI XUE, Dezhen/A-6062-2010; Ding, Xiangdong/K-4971-2013; Ren, Xiaobing/B-6072-2009 OI XUE, Dezhen/0000-0001-6132-1236; Ding, Xiangdong/0000-0002-1220-3097; Ren, Xiaobing/0000-0002-4973-2486 FU National Basic Research Program of China [2012CB619401]; National Natural Science Foundation of China [51302209, 51207121, 51431007, 51201126, 51320105014, 51321003]; 111 project of China [B06025]; LDRD program at Los ALamos National Laboratory FX The authors gratefully acknowledge the support of National Basic Research Program of China (Grant No. 2012CB619401), the National Natural Science Foundation of China (Grant Nos. 51302209, 51207121, 51431007, 51201126, 51320105014, and 51321003), and 111 project of China (B06025). We are also grateful to the LDRD program at Los ALamos National Laboratory for support. NR 44 TC 7 Z9 7 U1 6 U2 56 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAR 28 PY 2015 VL 117 IS 12 AR 124107 DI 10.1063/1.4916713 PG 7 WC Physics, Applied SC Physics GA CF1OJ UT WOS:000352315700030 ER PT J AU Schacht, M Danielson, JR Rahaman, S Torgerson, JR Zhang, J Schauer, MM AF Schacht, M. Danielson, J. R. Rahaman, S. Torgerson, J. R. Zhang, J. Schauer, M. M. TI Yb-171(+) 5D(3/2) hyperfine state detection and F=2 lifetime SO JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS LA English DT Article DE atomic state lifetimes; ion trapping; ytterbium ID FREQUENCY STANDARD; SINGLE-ION; TRANSITION AB We report on measurements of the lifetime of the 5D(3/2)(F= 2) state in single Yb-171 ions confined in a radiofrequency quadrupole trap. Experimental parameters that affect Yb-171 5D(3/2) hyperfine state preparation and detection efficiency are characterized and optimized. A set of wait times for optimal sampling of the D-3/2(F = 2) lifetime is chosen and used to measure that lifetime with high statistical sensitivity. A systematic variation in this lifetime seems to be apparent. The source of the variation was not identified, but ion number and cooling rate appear to be ruled out. A net determination is made of tau = 61.8 +/- (0.6)(stat) +/- (6.4)(sys) ms which is significantly longer than other measurements of the same quantity with four times better statistical precision than the most recent measurement. An alternate shelving scheme is proposed that would provide S-D state discrimination for Yb+ even isotopes as well as improved sensitivity for D state hyperfine discrimination in odd isotopes. C1 [Schacht, M.; Danielson, J. R.; Zhang, J.; Schauer, M. M.] Los Alamos Natl Lab, Div Phys, Los Alamos, NM 87545 USA. [Rahaman, S.] Georgia Inst Technol, Atlanta, GA 30332 USA. [Torgerson, J. R.] Quantel USA, Bozeman, MT 59715 USA. RP Schacht, M (reprint author), Los Alamos Natl Lab, Div Phys, P-23,Mail Stop H803, Los Alamos, NM 87545 USA. EM mschacht@lanl.gov RI Schacht, Mike/J-4441-2015 OI Schacht, Mike/0000-0002-5139-1369 FU Laboratory Directed Research and Development program at Los Alamos National Laboratory; NNSA US Department of Energy [DE-AC52-06NA25396] FX This work was supported by the Laboratory Directed Research and Development program at Los Alamos National Laboratory, operated by Los Alamos National Security, LLC for the NNSA US Department of Energy under contract No. DE-AC52-06NA25396 NR 23 TC 0 Z9 0 U1 1 U2 8 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-4075 EI 1361-6455 J9 J PHYS B-AT MOL OPT JI J. Phys. B-At. Mol. Opt. Phys. PD MAR 28 PY 2015 VL 48 IS 6 AR 065003 DI 10.1088/0953-4075/48/6/065003 PG 9 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA CD2FJ UT WOS:000350889800006 ER PT J AU Gogoi, MM Babu, SS Jayachandran, V Moorthy, KK Satheesh, SK Naja, M Kotamarthi, VR AF Gogoi, Mukunda M. Babu, S. Suresh Jayachandran, V. Moorthy, K. Krishna Satheesh, S. K. Naja, Manish Kotamarthi, V. R. TI Optical properties and CCN activity of aerosols in a high-altitude Himalayan environment: Results from RAWEX-GVAX SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article DE aerosol; scattering coefficient; absorption coefficient; cloud condensation nuclei ID CLOUD CONDENSATION NUCLEI; INDO-GANGETIC BASIN; MINERAL DUST; ATMOSPHERIC AEROSOLS; HYGROSCOPIC BEHAVIOR; ABSORBING AEROSOLS; SIZE DISTRIBUTION; LIGHT-ABSORPTION; WATER NUCLEATION; MANORA PEAK AB The seasonality and mutual dependence of aerosol optical properties and cloud condensation nuclei (CCN) activity under varying meteorological conditions at the high-altitude Nainital site (2km) in the Indo-Gangetic Plains were examined using nearly year-round measurements (June 2011 to March 2012) at the Atmospheric Radiation Measurement mobile facility as part of the Regional Aerosol Warming Experiment-Ganges Valley Aerosol Experiment of the Indian Space Research Organization and the U.S. Department of Energy. The results from collocated measurements provided enhanced aerosol scattering and absorption coefficients, CCN concentrations, and total condensation nuclei concentrations during the dry autumn and winter months. The CCN concentration (at a supersaturation of 0.46) was higher during the periods of high aerosol absorption (single scattering albedo (SSA)<0.80) than during the periods of high aerosol scattering (SSA>0.85), indicating that the aerosol composition seasonally changes and influences the CCN activity. The monthly mean CCN activation ratio (at a supersaturation of 0.46) was highest (>0.7) in late autumn (November); this finding is attributed to the contribution of biomass-burning aerosols to CCN formation at high supersaturation conditions. C1 [Gogoi, Mukunda M.; Babu, S. Suresh; Jayachandran, V.] Vikram Sarabhai Space Ctr, Space Phys Lab, Thiruvananthapuram, Kerala, India. [Moorthy, K. Krishna] Indian Space Res Org Head Quarters, Bangalore, Karnataka, India. [Satheesh, S. K.] Indian Inst Sci, Ctr Atmospher & Ocean Sci, Bangalore 560012, Karnataka, India. [Naja, Manish] Aryabhatta Res Inst Observat Sci, Naini Tal, India. [Kotamarthi, V. R.] Argonne Natl Lab, Div Environm Res, Argonne, IL 60439 USA. RP Babu, SS (reprint author), Vikram Sarabhai Space Ctr, Space Phys Lab, Thiruvananthapuram, Kerala, India. EM s_sureshbabu@vssc.gov.in RI Babu, Sudarsanam/D-1694-2010; OI Babu, Sudarsanam/0000-0002-3531-2579; Moorthy, K. Krishna/0000-0002-7234-3868 NR 89 TC 4 Z9 4 U1 2 U2 16 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD MAR 27 PY 2015 VL 120 IS 6 BP 2453 EP 2469 DI 10.1002/2014JD022966 PG 17 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA CG1UZ UT WOS:000353061800019 ER PT J AU Vugrin, ED Rostron, BL Verzi, SJ Brodsky, NS Brown, TJ Choiniere, CJ Coleman, BN Paredes, A Apelberg, BJ AF Vugrin, Eric D. Rostron, Brian L. Verzi, Stephen J. Brodsky, Nancy S. Brown, Theresa J. Choiniere, Conrad J. Coleman, Blair N. Paredes, Antonio Apelberg, Benjamin J. TI Modeling the Potential Effects of New Tobacco Products and Policies: A Dynamic Population Model for Multiple Product Use and Harm SO PLOS ONE LA English DT Article ID SMOKING-ATTRIBUTABLE MORTALITY; SIMSMOKE SIMULATION-MODEL; UNITED-STATES; REDUCING SMOKING; PUBLIC-POLICIES; PREVALENCE; DEATHS; CESSATION; IMPACT; PREVENTION AB Background Recent declines in US cigarette smoking prevalence have coincided with increases in use of other tobacco products. Multiple product tobacco models can help assess the population health impacts associated with use of a wide range of tobacco products. Methods and Findings We present a multi-state, dynamical systems population structure model that can be used to assess the effects of tobacco product use behaviors on population health. The model incorporates transition behaviors, such as initiation, cessation, switching, and dual use, related to the use of multiple products. The model tracks product use prevalence and mortality attributable to tobacco use for the overall population and by sex and age group. The model can also be used to estimate differences in these outcomes between scenarios by varying input parameter values. We demonstrate model capabilities by projecting future cigarette smoking prevalence and smoking-attributable mortality and then simulating the effects of introduction of a hypothetical new lower-risk tobacco product under a variety of assumptions about product use. Sensitivity analyses were conducted to examine the range of population impacts that could occur due to differences in input values for product use and risk. We demonstrate that potential benefits from cigarette smokers switching to the lower-risk product can be offset over time through increased initiation of this product. Model results show that population health benefits are particularly sensitive to product risks and initiation, switching, and dual use behaviors. Conclusion Our model incorporates the variety of tobacco use behaviors and risks that occur with multiple products. As such, it can evaluate the population health impacts associated with the introduction of new tobacco products or policies that may result in product switching or dual use. Further model development will include refinement of data inputs for non-cigarette tobacco products and inclusion of health outcomes such as morbidity and disability. C1 [Vugrin, Eric D.; Brodsky, Nancy S.] Sandia Natl Labs, Resilience & Regulatory Effects, Albuquerque, NM 87185 USA. [Rostron, Brian L.; Choiniere, Conrad J.; Coleman, Blair N.; Paredes, Antonio; Apelberg, Benjamin J.] US FDA, Ctr Tobacco Prod, Silver Spring, MD USA. [Verzi, Stephen J.] Sandia Natl Labs, Syst Res Anal & Applicat, Albuquerque, NM 87185 USA. [Brown, Theresa J.] Sandia Natl Labs, Policy & Decis Analyt, Albuquerque, NM 87185 USA. RP Vugrin, ED (reprint author), Sandia Natl Labs, Resilience & Regulatory Effects, POB 5800, Albuquerque, NM 87185 USA. EM edvugri@sandia.gov FU U.S. Food and Drug Administration through U.S. Department of Energy/Sandia National Laboratories [224109011]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was funded by the U.S. Food and Drug Administration through a contract with the U.S. Department of Energy/Sandia National Laboratories (funding document 224109011). Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. The funders, other than employees named as authors or described in the acknowledgments, had no role in the study design, data collection and analysis, decision to publish, or preparation of the manuscript. This article represents the views of the authors, and should not be construed to represent U.S. Food and Drug Administration's views or policies. NR 59 TC 6 Z9 6 U1 2 U2 3 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAR 27 PY 2015 VL 10 IS 3 AR e0121008 DI 10.1371/journal.pone.0121008 PG 26 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CE8ZT UT WOS:000352133600058 PM 25815840 ER PT J AU Song, JX Gordin, ML Xu, T Chen, SR Yu, ZX Sohn, H Lu, J Ren, Y Duan, YH Wang, DH AF Song, Jiangxuan Gordin, Mikhail L. Xu, Terrence Chen, Shuru Yu, Zhaoxin Sohn, Hiesang Lu, Jun Ren, Yang Duan, Yuhua Wang, Donghai TI Strong Lithium Polysulfide Chemisorption on Electroactive Sites of Nitrogen-Doped Carbon Composites For High-Performance Lithium-Sulfur Battery Cathodes SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE carbon materials; chemisorption; doping; electrochemistry; lithium-sulfur batteries ID ELECTROCHEMICAL PERFORMANCE; ELECTROLYTE AB Despite the high theoretical capacity of lithium-sulfur batteries, their practical applications are severely hindered by a fast capacity decay, stemming from the dissolution and diffusion of lithium polysulfides in the electrolyte. A novel functional carbon composite (carbon-nanotube-interpenetrated mesoporous nitrogen-doped carbon spheres, MNCS/CNT), which can strongly adsorb lithium polysulfides, is now reported to act as a sulfur host. The nitrogen functional groups of this composite enable the effective trapping of lithium polysulfides on electroactive sites within the cathode, leading to a much improved electrochemical performance (1200 mAh g(-1) after 200 cycles). The enhancement in adsorption can be attributed to the chemical bonding of lithium ions by nitrogen functional groups in the MNCS/CNT framework. Furthermore, the micrometer-sized spherical structure of the material yields a high areal capacity (ca. 6 mAh cm(-2)) with a high sulfur loading of approximately 5 mg cm(-2), which is ideal for practical applications of the lithium-sulfur batteries. C1 [Song, Jiangxuan; Gordin, Mikhail L.; Xu, Terrence; Chen, Shuru; Yu, Zhaoxin; Sohn, Hiesang; Wang, Donghai] Penn State Univ, Dept Mech & Nucl Engn, University Pk, PA 16802 USA. [Lu, Jun] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Ren, Yang] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. [Duan, Yuhua] US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. RP Wang, DH (reprint author), Penn State Univ, Dept Mech & Nucl Engn, University Pk, PA 16802 USA. EM dwang@psu.edu RI Duan, Yuhua/D-6072-2011; Song, Jiangxuan/G-8536-2015; Wang, Donghai/L-1150-2013 OI Duan, Yuhua/0000-0001-7447-0142; Wang, Donghai/0000-0001-7261-8510 FU Office of Vehicle Technologies of the U.S. Department of Energy (DOE) [DE-EE0005475]; U.S. DOE Office of Science [DE-AC02-06CH11357]; DOE Office of Energy Efficiency and Renewable Energy (EERE) Postdoctoral Research Award under EERE Vehicles Technology Program [DE-AC05-06OR23100] FX This work was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy (DOE; DE-EE0005475). Use of the Advanced Photon Source (APS) at Argonne National Laboratory was supported by the U.S. DOE Office of Science (DE-AC02-06CH11357). J.L. was supported by a DOE Office of Energy Efficiency and Renewable Energy (EERE) Postdoctoral Research Award under the EERE Vehicles Technology Program administered by the Oak Ridge Institute for Science and Education for the DOE (DE-AC05-06OR23100). NR 28 TC 145 Z9 147 U1 81 U2 379 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD MAR 27 PY 2015 VL 54 IS 14 BP 4325 EP 4329 DI 10.1002/anie.201411109 PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA CE2VW UT WOS:000351679600032 PM 25663183 ER PT J AU Filippova, EV Kuhn, ML Osipiuk, J Kiryukhina, O Joachimiak, A Ballicora, MA Anderson, WF AF Filippova, Ekaterina V. Kuhn, Misty L. Osipiuk, Jerzy Kiryukhina, Olga Joachimiak, Andrzej Ballicora, Miguel A. Anderson, Wayne F. TI A Novel Polyamine Allosteric Site of SpeG from Vibrio cholerae Is Revealed by Its Dodecameric Structure SO JOURNAL OF MOLECULAR BIOLOGY LA English DT Article DE spermidine/spermine; dodecamer; allosteric enzyme; GNAT; acetyltransferase ID GCN5-RELATED N-ACETYLTRANSFERASES; X-RAY CRYSTALLOGRAPHY; PROTEIN DATA-BANK; ESCHERICHIA-COLI; SPERMIDINE ACETYLTRANSFERASE; HIGH-THROUGHPUT; MOLECULAR-GRAPHICS; GNAT SUPERFAMILY; MODEL; INHIBITION AB Spermidine N-acetyltransferase, encoded by the gene speG, catalyzes the initial step in the degradation of polyamines and is a critical enzyme for determining the polyamine concentrations in bacteria. In Escherichia coli, studies have shown that SpeG is the enzyme responsible for acetylating spermidine under stress conditions and for preventing spermidine toxicity. Not all bacteria contain speG, and many bacterial pathogens have developed strategies to either acquire or silence it for pathogenesis. Here, we present thorough kinetic analyses combined with structural characterization of the VCA0947 SpeG enzyme from the important human pathogen Vibrio cholerae. Our studies revealed the unexpected presence of a previously unknown allosteric site and an unusual dodecameric structure for a member of the Gcn5-related N-acetyltransferase superfamily. We show that SpeG forms dodecamers in solution and in crystals and describe its three-dimensional structure in several ligand-free and liganded structures. Importantly, these structural data define the first view of a polyamine bound in an allosteric site of an N-acetyltransferase. Kinetic characterization of SpeG from V. cholerae showed that it acetylates spermidine and spermine. The behavior of this enzyme is complex and exhibits sigmoidal curves and substrate inhibition. We performed a detailed non-linear regression kinetic analysis to simultaneously fit families of substrate saturation curves to uncover a simple kinetic mechanism that explains the apparent complexity of this enzyme. Our results provide a fundamental understanding of the bacterial SpeG enzyme, which will be key toward understanding the regulation of polyamine levels in bacteria during pathogenesis. (C) 2015 The Authors. Published by Elsevier Ltd. This is an open access article under the CC BY-NC-ND license (http://creativecommons.org/licenses/by-nc-nd/4.0/). C1 [Filippova, Ekaterina V.; Kuhn, Misty L.; Kiryukhina, Olga; Anderson, Wayne F.] Northwestern Univ, Feinberg Sch Med, Dept Biochem & Mol Genet, Ctr Struct Genom Infect Dis, Chicago, IL 60611 USA. [Osipiuk, Jerzy; Joachimiak, Andrzej] Argonne Natl Lab, Biosci Div, Argonne, IL 60439 USA. [Ballicora, Miguel A.] Loyola Univ, Dept Chem & Biochem, Chicago, IL 60626 USA. RP Anderson, WF (reprint author), Northwestern Univ, Feinberg Sch Med, Dept Biochem & Mol Genet, 303 East Chicago Ave,Mail Code S215, Chicago, IL 60611 USA. EM wf-anderson@northwestern.edu FU U.S. Department of Energy [DE-AC02-06CH11357]; National Institute of Allergy and Infectious Diseases, National Institutes of Health, Department of Health and Human Services [HHSN272200700058C, HHSN272201200026C]; National Science Foundation [MCB 1024945] FX We would like to extend our sincere appreciation to Samuel Light for his critical review of the manuscript and to Ludmilla Shuvalova and George Minasov for their helpful discussions. Additionally, we would like to thank Lour Volkart and Min Zhou at Argonne National Laboratory for their technical assistance. We would also like to thank the Keck Biophysics Facility at Northwestern University (Evanston Campus) for their assistance with ITC data collection and processing. The data collection for determining crystal structures presented in this manuscript was performed at the LS-CAT and SBC-CAT beamlines at the Advanced Photon Source Science User Facility operated for the U.S. Department of Energy and supported by the U.S. Department of Energy under Contract No. DE-AC02-06CH11357. This project has been funded in whole or in part with federal funds from the National Institute of Allergy and Infectious Diseases, National Institutes of Health, Department of Health and Human Services, under Contracts No. HHSN272200700058C and HHSN272201200026C (W.F.A.), and from the National Science Foundation grant MCB 1024945 (M.A.B.). NR 55 TC 6 Z9 6 U1 1 U2 8 PU ACADEMIC PRESS LTD- ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL RD, LONDON NW1 7DX, ENGLAND SN 0022-2836 EI 1089-8638 J9 J MOL BIOL JI J. Mol. Biol. PD MAR 27 PY 2015 VL 427 IS 6 BP 1316 EP 1334 DI 10.1016/j.jmb.2015.01.009 PN B PG 19 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CE4KE UT WOS:000351798700008 PM 25623305 ER PT J AU Jarrige, I Kotani, A Yamaoka, H Tsujii, N Ishii, K Upton, M Casa, D Kim, J Gog, T Hancock, JN AF Jarrige, I. Kotani, A. Yamaoka, H. Tsujii, N. Ishii, K. Upton, M. Casa, D. Kim, J. Gog, T. Hancock, J. N. TI Kondo Interactions from Band Reconstruction in YbInCu4 SO PHYSICAL REVIEW LETTERS LA English DT Article ID 1ST-ORDER VALENCE TRANSITION; ELECTRONIC-STRUCTURE; PHASE-TRANSITION; IMPURITY MODEL; YBIN1-XAGXCU4; PHOTOEMISSION; LUINCU4; SPECTRA; YBXCU4; AU AB We combine resonant inelastic x-ray scattering and model calculations in the Kondo lattice compound YbInCu4, a system characterized by a dramatic increase in Kondo temperature and associated valence fluctuations below a first-order valence transition at T congruent to 42 K. The bulk-sensitive, element-specific, and valence-projected charge excitation spectra reveal an unusual quasigap in the Yb-derived state density which drives an instability of the electronic structure and renormalizes the low-energy effective Hamiltonian at the transition. Our results provide long-sought experimental evidence for a link between temperature-driven changes in the low-energy Kondo scale and the higher-energy electronic structure of this system. C1 [Jarrige, I.] Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA. [Kotani, A.] High Energy Accelerator Res Org, Inst Mat Struct Sci, Photon Factory, Tsukuba, Ibaraki 3050801, Japan. [Yamaoka, H.] RIKEN SPring 8 Ctr, Sayo, Hyogo 6795148, Japan. [Tsujii, N.] Natl Inst Mat Sci, Quantum Beam Ctr, Tsukuba, Ibaraki 3050047, Japan. [Ishii, K.] Japan Atom Energy Agcy, SPring 8, Sayo, Hyogo 6795148, Japan. [Upton, M.; Casa, D.; Kim, J.; Gog, T.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Hancock, J. N.] Univ Connecticut, Dept Phys, Storrs, CT 06269 USA. [Hancock, J. N.] Univ Connecticut, Inst Mat Sci, Storrs, CT 06269 USA. RP Jarrige, I (reprint author), Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA. EM jarrige@bnl.gov RI Casa, Diego/F-9060-2016; Jarrige, Ignace/M-6371-2016; Tsujii, Naohito/H-2544-2011 OI Jarrige, Ignace/0000-0002-1043-5695; Tsujii, Naohito/0000-0002-6181-5911 FU US DOE [DE-AC02-06CH11357] FX We thank T. Fukuda for his help with aligning the single crystal. Use of the APS, an Office of Science User Facility operated for the US DOE Office of Science by Argonne National Laboratory, was supported by the US DOE under Contract No. DE-AC02-06CH11357. NR 29 TC 2 Z9 2 U1 3 U2 22 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 27 PY 2015 VL 114 IS 12 AR 126401 DI 10.1103/PhysRevLett.114.126401 PG 5 WC Physics, Multidisciplinary SC Physics GA CE3OG UT WOS:000351735600013 PM 25860761 ER PT J AU Mounce, AM Yasuoka, H Koutroulakis, G Ni, N Bauer, ED Ronning, F Thompson, JD AF Mounce, A. M. Yasuoka, H. Koutroulakis, G. Ni, N. Bauer, E. D. Ronning, F. Thompson, J. D. TI Detection of a Spin-Triplet Superconducting Phase in Oriented Polycrystalline U2PtC2 Samples Using Pt-195 Nuclear Magnetic Resonance SO PHYSICAL REVIEW LETTERS LA English DT Article ID KNIGHT-SHIFT; CRITICAL-FIELD; UPT3; FERROMAGNETISM; COEXISTENCE; RELAXATION; DEPENDENCE; STATE AB Nuclear magnetic resonance (NMR) measurements on the Pt-195 nucleus in an aligned powder of the moderately heavy-fermion material U 2PtC2 are consistent with spin- triplet pairing in its superconducting state. Across the superconducting transition temperature and to much lower temperatures, the NMR Knight shift is temperature independent for field both parallel and perpendicular to the tetragonal c axis, expected for triplet equal-spin pairing superconductivity. The NMR spin-lattice relaxation rate 1/T-1, in the normal state, exhibits characteristics of ferromagnetic fluctuations, compatible with an enhanced Wilson ratio. In the superconducting state, 1/T-1 follows a power law with temperature without a coherence peak giving additional support that U2PtC2 is an unconventional superconductor. Bulk measurements of the ac susceptibility and resistivity indicate that the upper critical field exceeds the Pauli limiting field for spin-singlet pairing and is near the orbital limiting field, an additional indication for spin- triplet pairing. C1 [Mounce, A. M.; Yasuoka, H.; Koutroulakis, G.; Ni, N.; Bauer, E. D.; Ronning, F.; Thompson, J. D.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Mounce, AM (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. OI Ronning, Filip/0000-0002-2679-7957; Bauer, Eric/0000-0003-0017-1937 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; Los Alamos LDRD program FX We thank J. M. Lawrence for useful discussion. Work at Los Alamos was performed under the auspices of the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. A. M., G. K., and N. N. would also like to acknowledge postdoctoral fellowships funded by the Los Alamos LDRD program. NR 30 TC 3 Z9 3 U1 2 U2 19 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 27 PY 2015 VL 114 IS 12 DI 10.1103/PhysRevLett.114.127001 PG 5 WC Physics, Multidisciplinary SC Physics GA CE3OG UT WOS:000351735600015 PM 25860768 ER PT J AU Kelly, PL Filippenko, AV Burke, DL Hicken, M Ganeshalingam, M Zheng, WK AF Kelly, Patrick L. Filippenko, Alexei V. Burke, David L. Hicken, Malcolm Ganeshalingam, Mohan Zheng, WeiKang TI Distances with < 4% precision from type Ia supernovae in young star-forming environments SO SCIENCE LA English DT Article ID LIGHT-CURVE SHAPES; H-ALPHA; ABSOLUTE MAGNITUDES; HUBBLE RESIDUALS; HOST GALAXIES; LUMINOSITIES; ULTRAVIOLET; EXTINCTION; REGRESSION; MORPHOLOGY AB The luminosities of type Ia supernovae (SNe), the thermonuclear explosions of white-dwarf stars, vary systematically with their intrinsic color and the rate at which they fade. From images taken with the Galaxy Evolution Explorer (GALEX), we identified SNe Ia that erupted in environments that have high ultraviolet surface brightness and star-formation surface density. When we apply a steep model extinction law, we calibrate these SNe using their broadband optical light curves to within similar to 0.065 to 0.075 magnitude, corresponding to <4% in distance. The tight scatter, probably arising from a small dispersion among progenitor ages, suggests that variation in only one progenitor property primarily accounts for the relationship between their light-curve widths, colors, and luminosities. C1 [Kelly, Patrick L.; Filippenko, Alexei V.; Zheng, WeiKang] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. [Burke, David L.] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Hicken, Malcolm] Harvard Smithsonian Ctr Astrophys, Cambridge, MA 02138 USA. [Ganeshalingam, Mohan] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Kelly, PL (reprint author), Univ Calif Berkeley, Dept Astron, 601 Campbell Hall, Berkeley, CA 94720 USA. EM pkelly@astro.berkeley.edu FU Christopher R. Redlich Fund; TABASGO Foundation; NSF [AST-1211916]; SLAC Department of Energy [DE-AC02-76SF00515] FX We thank S. Sim, J. C. Wheeler, J. Silverman, A. Conley, M. Graham, D. Kasen, I. Shivvers, and R. Kessler for useful discussions and comments on the paper and J. Schwab for his help providing background about theoretical modeling. We are grateful to the staffs at Lick Observatory and Kitt Peak National Observatory (KPNO) for their assistance. The late Weidong Li was instrumental to the success of LOSS. A.V.F.'s supernova group at the University of California Berkeley has received generous financial assistance from the Christopher R. Redlich Fund, the TABASGO Foundation, and NSF grant AST-1211916. The Katzman Automatic Imaging Telescope and its ongoing operation were made possible by donations from Sun Microsystems, the Hewlett-Packard Company, AutoScope Corporation, Lick Observatory, NSF, the University of California, the Sylvia and Jim Katzman Foundation, and the TABASGO Foundation. The SLAC Department of Energy contract number is DE-AC02-76SF00515. GALEX data are available from http://galex.stsci.edu/GR6/, SDSS data may be obtained at www.sdss.org, the KPNO imaging is archived at http://portal-nvo.noao.edu, and the Lick Observatory images are available from http://astro.berkeley.edu/bait/public_html/iahostpaper/. NR 35 TC 13 Z9 13 U1 0 U2 1 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD MAR 27 PY 2015 VL 347 IS 6229 BP 1459 EP 1462 DI 10.1126/science.1261475 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CE9AT UT WOS:000352136400036 PM 25814580 ER PT J AU Byrne, JM Klueglein, N Pearce, C Rosso, KM Appel, E Kappler, A AF Byrne, James M. Klueglein, Nicole Pearce, Carolyn Rosso, Kevin M. Appel, Erwin Kappler, Andreas TI Redox cycling of Fe(II) and Fe(III) in magnetite by Fe-metabolizing bacteria SO SCIENCE LA English DT Article ID PALUSTRIS STRAIN TIE-1; NANOPARTICULATE MAGNETITE; FE3-XTIXO4 NANOPARTICLES; ELECTRON-TRANSFER; REDUCTION; OXIDATION; IRON; STOICHIOMETRY; OXIDE AB Microorganisms are a primary control on the redox-induced cycling of iron in the environment. Despite the ability of bacteria to grow using both Fe(II) and Fe(III) bound in solid-phase iron minerals, it is currently unknown whether changing environmental conditions enable the sharing of electrons in mixed-valent iron oxides between bacteria with different metabolisms. We show through magnetic and spectroscopic measurements that the phototrophic Fe(II)-oxidizing bacterium Rhodopseudomonas palustris TIE-1 oxidizes magnetite (Fe3O4) nanoparticles using light energy. This process is reversible in co-cultures by the anaerobic Fe(III)-reducing bacterium Geobacter sulfurreducens. These results demonstrate that Fe ions bound in the highly crystalline mineral magnetite are bioavailable as electron sinks and electron sources under varying environmental conditions, effectively rendering magnetite a naturally occurring battery. C1 [Byrne, James M.; Klueglein, Nicole; Kappler, Andreas] Univ Tubingen, Ctr Appl Geosci, Geomicrobiol, D-72076 Tubingen, Germany. [Pearce, Carolyn] Univ Manchester, Sch Chem, Manchester M13 9PL, Lancs, England. [Pearce, Carolyn; Rosso, Kevin M.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Appel, Erwin] Univ Tubingen, Ctr Appl Geosci, Geophys, D-72076 Tubingen, Germany. RP Byrne, JM (reprint author), Univ Tubingen, Ctr Appl Geosci, Geomicrobiol, Sigwartstr 10, D-72076 Tubingen, Germany. EM James.Byrne@uni-tuebingen.de RI Kappler, Andreas/G-7221-2016; Byrne, James/L-4860-2016 OI Byrne, James/0000-0002-4399-7336 FU Deutsche Forschungsgemeinschaft; Pacific Northwest National Laboratory Science Focus Area, the Subsurface Biogeochemical Research program of the U.S. Department of Energy Office of Biological and Environmental Research FX We thank G. Ojha for help with kappa-T measurements and C. Berthold for advice on mu-XRD. This work was funded by the Deutsche Forschungsgemeinschaft. Part of this work was funded by the Pacific Northwest National Laboratory Science Focus Area, the Subsurface Biogeochemical Research program of the U.S. Department of Energy Office of Biological and Environmental Research. We thank J. Liu (Peking University) for providing TEM images, which were taken in the Environmental Molecular Science Laboratory (EMSL), a national user facility supported by the OBER and located at PNNL. All data associated with this publication are available at www.pangaea.de. NR 25 TC 24 Z9 25 U1 34 U2 197 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD MAR 27 PY 2015 VL 347 IS 6229 BP 1473 EP 1476 DI 10.1126/science.aaa4834 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CE9AT UT WOS:000352136400040 PM 25814583 ER PT J AU Lindsay, L Broido, DA Carrete, J Mingo, N Reinecke, TL AF Lindsay, L. Broido, D. A. Carrete, Jesus Mingo, Natalio Reinecke, T. L. TI Anomalous pressure dependence of thermal conductivities of large mass ratio compounds SO PHYSICAL REVIEW B LA English DT Article ID PHASE-TRANSFORMATION; MAGNESIUM OXIDE; PHONONS; AMORPHIZATION; CRYSTALS; EQUATION; MGO AB The lattice thermal conductivities (kappa) of binary compound materials are examined as a function of hydrostatic pressure P using a first-principles approach. Compounds with relatively small mass ratios, such as MgO, show an increase in kappa with P, consistent with measurements. Conversely, compounds with large mass ratios that create significant frequency gaps between acoustic and optic phonons (e.g., BSb, BAs, BeTe, BeSe) exhibit decreasing. with increasing P, a behavior that cannot be understood using simple theories of kappa. This anomalous P dependence of kappa arises from the fundamentally different nature of the intrinsic scattering processes for heat-carrying acoustic phonons in large mass ratio compounds compared to those with small mass ratios. This work demonstrates the power of first-principles methods for thermal properties and advances a broad paradigm for understanding thermal transport in nonmetals. C1 [Lindsay, L.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Broido, D. A.] Boston Coll, Dept Phys, Chestnut Hill, MA 02467 USA. [Carrete, Jesus; Mingo, Natalio] CEA Grenoble, LITEN, F-38054 Grenoble 9, France. [Reinecke, T. L.] Naval Res Lab, Washington, DC 20375 USA. RP Lindsay, L (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RI Lindsay, Lucas/C-9221-2012; Carrete Montana, Jesus/G-9490-2012 OI Lindsay, Lucas/0000-0001-9645-7993; Carrete Montana, Jesus/0000-0003-0971-1098 FU National Science Foundation [1402949]; ONR [N00014-13-1-0234]; Institut Carnot through project SIEVE; DARPA; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division FX L.L. acknowledges support from the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division for work done at ORNL. D.A.B. acknowledges support from the National Science Foundation under Grant No. 1402949 and from ONR under Grant No. N00014-13-1-0234. N.M. and J.C. acknowledge support from Institut Carnot through project SIEVE. T.L.R. acknowledges support from ONR and DARPA. We thank David Cahill and Greg Hohensee for providing the impurity concentrations in their MgO sample. We also thank Saikat Mukhopadhyay and Derek Stewart for kindly providing us with their calculated anharmonic IFCs for BN. NR 43 TC 7 Z9 7 U1 5 U2 36 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAR 27 PY 2015 VL 91 IS 12 AR 121202 DI 10.1103/PhysRevB.91.121202 PG 5 WC Physics, Condensed Matter SC Physics GA CE3NK UT WOS:000351733100001 ER PT J AU Basharin, AA Kafesaki, M Economou, EN Soukoulis, CM Fedotov, VA Savinov, V Zheludev, NI AF Basharin, Alexey A. Kafesaki, Maria Economou, Eleftherios N. Soukoulis, Costas M. Fedotov, Vassili A. Savinov, Vassili Zheludev, Nikolay I. TI Dielectric Metamaterials with Toroidal Dipolar Response SO PHYSICAL REVIEW X LA English DT Article ID MOMENT; ELECTRODYNAMICS; GENERATION; CRYSTALS; SURFACE; STATE; FIELD; RING AB Toroidal multipoles are the terms missing in the standard multipole expansion; they are usually overlooked due to their relatively weak coupling to the electromagnetic fields. Here, we propose and theoretically study all-dielectric metamaterials of a special class that represent a simple electromagnetic system supporting toroidal dipolar excitations in the THz part of the spectrum. We show that resonant transmission and reflection of such metamaterials is dominated by toroidal dipole scattering, the neglect of which would result in a misunderstanding interpretation of the metamaterials' macroscopic response. Because of the unique field configuration of the toroidal mode, the proposed metamaterials could serve as a platform for sensing or enhancement of light absorption and optical nonlinearities. C1 [Basharin, Alexey A.; Kafesaki, Maria; Economou, Eleftherios N.; Soukoulis, Costas M.] Fdn Res & Technol Hellas FORTH, IESL, Iraklion 71110, Greece. [Basharin, Alexey A.] Natl Res Univ, Moscow Power Engn Inst, Moscow 112250, Russia. [Kafesaki, Maria] Univ Crete, Dept Mat Sci & Technol, Iraklion 71003, Greece. [Economou, Eleftherios N.] Univ Crete, Dept Phys, Iraklion 71003, Greece. [Soukoulis, Costas M.] Iowa State Univ, USDOE, Ames Lab, Ames, IA 50011 USA. [Soukoulis, Costas M.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Fedotov, Vassili A.; Savinov, Vassili; Zheludev, Nikolay I.] Univ Southampton, Optoelect Res Ctr, Southampton SO17 1BJ, Hants, England. [Fedotov, Vassili A.; Savinov, Vassili; Zheludev, Nikolay I.] Univ Southampton, Ctr Photon Metamat, Southampton SO17 1BJ, Hants, England. [Zheludev, Nikolay I.] Nanyang Technol Univ, Ctr Disrupt Photon Technol, Singapore 637371, Singapore. RP Basharin, AA (reprint author), Fdn Res & Technol Hellas FORTH, IESL, POB 1385, Iraklion 71110, Greece. EM basharin@iesl.forth.gr RI Zheludev, Nikolay/C-2284-2014; Economou, Eleftherios /E-6374-2010; Metamaterials, Southampton/E-1171-2014; Soukoulis, Costas/A-5295-2008; Kafesaki, Maria/E-6843-2012; Savinov, Vassili/D-2417-2017; OI Zheludev, Nikolay/0000-0002-1013-6636; Kafesaki, Maria/0000-0002-9524-2576; Savinov, Vassili/0000-0001-7203-7222; Basharin, Alexey/0000-0003-0851-5642 FU EU projects ENSEMBLE and By-Nanoera; Greek project ERC-02 ExEL [6260]; Department of Energy (Basic Energy Sciences) [DE-AC02-07CH11358]; Russian Foundation for Basic Research [13-02-00732, 13-08-01278]; Russian Federal Program "Scientific and Scientific-Pedagogical Staff of Innovative Russia" [14.B37.21.1211]; Royal Society; U.K.'s Engineering and Physical Sciences Research Council under the Programme Grant on Photonic Metamaterials and Career Acceleration Fellowship; MOE Singapore [MOE2011-T3-1-005] FX The authors acknowledge the financial support by the EU projects ENSEMBLE and By-Nanoera and the Greek project ERC-02 ExEL (Grant No. 6260). Work at Ames Laboratory was partially supported by the Department of Energy (Basic Energy Sciences) under Contract No. DE-AC02-07CH11358 (computational studies). Work at the National Research University "Moscow Power Engineering Institute" was supported by the Russian Foundation for Basic Research (Grant Agreements No. 13-02-00732 and No. 13-08-01278) and the Russian Federal Program "Scientific and Scientific-Pedagogical Staff of Innovative Russia" for 2009-2013 (Agreement No. 14.B37.21.1211). V. A. F., V. S., and N. I. Z. acknowledge financial support of the Royal Society and the U.K.'s Engineering and Physical Sciences Research Council under the Programme Grant on Photonic Metamaterials and Career Acceleration Fellowship (V. A. F.). Work at Nanyang Technological University was partially supported by the MOE Singapore Grant No. MOE2011-T3-1-005. NR 62 TC 30 Z9 30 U1 10 U2 71 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2160-3308 J9 PHYS REV X JI Phys. Rev. X PD MAR 27 PY 2015 VL 5 IS 1 AR 011036 DI 10.1103/PhysRevX.5.011036 PG 11 WC Physics, Multidisciplinary SC Physics GA CE3OB UT WOS:000351735100001 ER PT J AU Veintemillas-Verdaguer, S Luengo, Y Serna, CJ Andres-Verges, M Varela, M Calero, M Lazaro-Carrillo, A Villanueva, A Sisniega, A Montesinos, P Morales, MP AF Veintemillas-Verdaguer, S. Luengo, Y. Serna, C. J. Andres-Verges, M. Varela, M. Calero, Macarena Lazaro-Carrillo, Ana Villanueva, Angeles Sisniega, A. Montesinos, P. Morales, M. P. TI Bismuth labeling for the CT assessment of local administration of magnetic nanoparticles SO NANOTECHNOLOGY LA English DT Article DE iron bismuth nanocrystals; surface modification; magnetic properties; radiopacity; computed tomography; magnetic resonance imaging ID RAY COMPUTED-TOMOGRAPHY; IN-VIVO; SULFIDE NANOPARTICLES; CONTRAST AGENTS; OXIDE NANOPARTICLES; POLYETHYLENE-GLYCOL; TOXICITY; IRON; CYTOTOXICITY; VITRO AB Many therapeutic applications of magnetic nanoparticles involve the local administration of nanometric iron oxide based materials as seeds for magnetothermia or drug carriers. A simple and widespread way of controlling the process using x-ray computed tomography (CT) scanners is desirable. The combination of iron and bismuth in one entity will increase the atenuation of x-rays, offering such a possibility. In order to check this possibility core-shell nanocrystals of iron oxide@bismuth oxide have been synthesized by an aqueous route and stabilized in water by polyethylene glycol (PEG), and we have evaluated their ability to generate contrast by CT and magnetic resonance imaging (MRI) to measure the radiopacity and proton relaxivities using phantoms. High-resolution scanning transmission electron microscopy (STEM) revealed that the material consists of a highly crystalline 8 nm core of maghemite and a 1 nm shell of bismuth atoms either isolated or clustered on the nanocrystal's surface. The comparison of mu CT and MRI images of mice acquired in the presence of the contrast shows that when local accumulations of the magnetic nanoparticles take place, CT images are more superior in the localization of the magnetic nanoparticles than MRI images, which results in magnetic field inhomogeneity artifacts. C1 [Veintemillas-Verdaguer, S.; Luengo, Y.; Serna, C. J.; Morales, M. P.] CSIC, Inst Ciencia Mat Madrid, Madrid 28049, Spain. [Andres-Verges, M.] Fac Ciencias UEX, Dept Quim Organ & Inorgan, Badajoz 06006, Spain. [Varela, M.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Varela, M.] Univ Complutense Madrid, Dept Fis Aplicada 3, E-28040 Madrid, Spain. [Varela, M.] Univ Complutense Madrid, Inst Pluridisciplinar, E-28040 Madrid, Spain. [Calero, Macarena; Lazaro-Carrillo, Ana; Villanueva, Angeles] Univ Autonoma Madrid, Dept Biol, E-28049 Madrid, Spain. [Calero, Macarena; Lazaro-Carrillo, Ana; Villanueva, Angeles] IMDEA Nanociencia, Madrid, Spain. [Sisniega, A.] Univ Carlos III Madrid, Dept Bioingn & Ingn Aerosp, E-28903 Getafe, Spain. [Montesinos, P.] IiSGM, Madrid, Spain. RP Veintemillas-Verdaguer, S (reprint author), CSIC, Inst Ciencia Mat Madrid, Sor Juana Ines de la Cruz 3, Madrid 28049, Spain. EM sabino@icmm.csic.es RI Varela, Maria/E-2472-2014; Lazaro-Carrillo, Ana/M-5714-2014; Morales Herrero, Maria del Puerto/A-4558-2011 OI Varela, Maria/0000-0002-6582-7004; Lazaro-Carrillo, Ana/0000-0002-7733-6114; Morales Herrero, Maria del Puerto/0000-0002-7290-7029 FU Spanish Ministry of Economy and Competitiveness [MAT2011-23641]; ERC Starting Investigator Award [STEMOX 739239]; Guerbet Group FX This work was supported by the Spanish Ministry of Economy and Competitiveness through Project MAT2011-23641. The authors acknowledge the help of Dr Ruiz Cabello and Dr Herranz in the relaxometric measurements at the Centro Nacional de Investigaciones Cardiovasculares CNIC and acknowledge Guerbet Group for the economic support and the supply of Xenetix (R). The research at ORNL US, the Department of Energy (DOE), Basic Energy Sciences (BES), the Materials Sciences and Energy Division (MV) and the Complutense University of Madrid (UCM) was supported by the ERC Starting Investigator Award STEMOX 739239. NR 48 TC 1 Z9 1 U1 3 U2 38 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 EI 1361-6528 J9 NANOTECHNOLOGY JI Nanotechnology PD MAR 27 PY 2015 VL 26 IS 13 AR 135101 DI 10.1088/0957-4484/26/13/135101 PG 10 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA CD2FP UT WOS:000350890700006 PM 25760138 ER PT J AU Green, DJ Shadman, M Jones, JC Frayo, SL Kenoyer, AL Hylarides, MD Hamlin, DK Wilbur, DS Balkan, ER Lin, YK Miller, BW Frost, SHL Gopal, AK Orozco, JJ Gooley, TA Laird, KL Till, BG Back, T Sandmaier, BM Pagel, JM Press, OW AF Green, Damian J. Shadman, Mazyar Jones, Jon C. Frayo, Shani L. Kenoyer, Aimee L. Hylarides, Mark D. Hamlin, Donald K. Wilbur, D. Scott Balkan, Ethan R. Lin, Yukang Miller, Brian W. Frost, Sofia H. L. Gopal, Ajay K. Orozco, Johnnie J. Gooley, Theodore A. Laird, Kelly L. Till, Brian G. Back, Tom Sandmaier, Brenda M. Pagel, John M. Press, Oliver W. TI Astatine-211 conjugated to an anti-CD20 monoclonal antibody eradicates disseminated B-cell lymphoma in a mouse model SO BLOOD LA English DT Article ID NON-HODGKINS-LYMPHOMA; IBRITUMOMAB TIUXETAN RADIOIMMUNOTHERAPY; BONE-MARROW-TRANSPLANTATION; POLYMERASE-CHAIN-REACTION; HIGH-DOSE THERAPY; FOLLICULAR LYMPHOMA; I-131 TOSITUMOMAB; ALPHA-CAMERA; LOW-GRADE; PRETARGETED RADIOIMMUNOTHERAPY AB alpha-Emitting radionuclides deposit a large amount of energy within a few cell diameters and may be particularly effective for radioimmunotherapy targeting minimal residual disease (MRD). To evaluate this hypothesis, At-211-labeled 1F5 monoclonal antibody (mAb) (anti-CD20) was studied in both bulky lymphoma tumor xenograft and MRD animal models. Superior treatment responses to At-211-labeled 1F5 mAb were evident in the MRD setting. Lymphoma xenograft tumor-bearing animals treatedwith doses of up to 48 mu Ci of At-211-labeled anti-CD20mAb ([At-211] 1F5-B10) experiencedmodest responses(0% cures but two- to three fold prolongation of survival compared with negative controls). In contrast, 70% of animals in the MRD lymphoma model demonstrated complete eradication of disease when treated with At-211-B-10-1F5 at a radiation dose that was less than one-third (15 mu Ci) of the highest dose given to xenograft animals. Tumor progression among untreated control animals in both models was uniformly lethal. After 130 days, no significant renal or hepatic toxicity was observed in the cured animals receiving 15 mu Ci of [At-211]1F5-B10. These findings suggest that a-emitters are highly efficacious in MRD settings, where isolated cells and small tumor clusters prevail. C1 [Green, Damian J.; Shadman, Mazyar; Jones, Jon C.; Frayo, Shani L.; Kenoyer, Aimee L.; Hylarides, Mark D.; Lin, Yukang; Frost, Sofia H. L.; Gopal, Ajay K.; Orozco, Johnnie J.; Gooley, Theodore A.; Laird, Kelly L.; Till, Brian G.; Sandmaier, Brenda M.; Pagel, John M.; Press, Oliver W.] Fred Hutchinson Canc Res Ctr, Div Clin Res, Seattle, WA 98109 USA. [Green, Damian J.; Shadman, Mazyar; Gopal, Ajay K.; Orozco, Johnnie J.; Till, Brian G.; Sandmaier, Brenda M.; Pagel, John M.; Press, Oliver W.] Univ Washington, Dept Med, Seattle, WA USA. [Hamlin, Donald K.; Wilbur, D. Scott; Balkan, Ethan R.] Univ Washington, Dept Radiat Oncol, Seattle, WA 98195 USA. [Miller, Brian W.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Back, Tom] Univ Gothenberg, Dept Radiat Phys, Gothenburg, Sweden. RP Green, DJ (reprint author), Fred Hutchinson Canc Res Ctr, Div Clin Res, 1100 Fairview Ave North,MS D3-190, Seattle, WA 98109 USA. EM dgreen@fhcrc.org FU National Institutes of Health, National Cancer Institute [K08CA151682, P01CA044991, R01CA076287, CA136639]; David and Patricia Giuliani Family Foundation; Leukemia and Lymphoma Society FX This work was supported by grants from the National Institutes of Health, National Cancer Institute (K08CA151682) (D.J.G.) (P01CA044991, R01CA076287, and CA136639) (O.W.P.) and the David and Patricia Giuliani Family Foundation (O.W.P.). A.K.G. is a Clinical Research Scholar of the Leukemia and Lymphoma Society. The authors express appreciation to L. Elizabeth Budde for generating the Granta-519 FFLuc cell line. NR 46 TC 4 Z9 4 U1 0 U2 8 PU AMER SOC HEMATOLOGY PI WASHINGTON PA 2021 L ST NW, SUITE 900, WASHINGTON, DC 20036 USA SN 0006-4971 EI 1528-0020 J9 BLOOD JI Blood PD MAR 26 PY 2015 VL 125 IS 13 BP 2111 EP 2119 DI 10.1182/blood-2014-11-612770 PG 9 WC Hematology SC Hematology GA CI3CX UT WOS:000354626300018 PM 25628467 ER PT J AU Aad, G Abbott, B Abdallah, J Khalek, SA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Agatonovic-Jovin, T Aguilar-Saavedra, JA Agustoni, M Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TPA Akimoto, G Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Allbrooke, BMM Allison, LJ Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA 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CA ATLAS Collaboration TI Search for Higgs and Z Boson Decays to J/psi gamma and Upsilon(nS)gamma with the ATLAS Detector SO PHYSICAL REVIEW LETTERS LA English DT Article ID HADRONIC Z(0) DECAYS; PHYSICS; COUPLINGS; PHOTON; LHC; PSI AB A search for the decays of the Higgs and Z bosons to J/psi gamma and Upsilon(nS)gamma (n = 1,2,3) is performed with pp collision data samples corresponding to integrated luminosities of up to 20.3 fb(-1) collected at root s = 8 TeV with the ATLAS detector at the CERN Large Hadron Collider. No significant excess of events is observed above expected backgrounds and 95% C.L. upper limits are placed on the branching fractions. In the J/psi gamma final state the limits are 1.5 x 10(-3) and 2.6 x 10(-6) for the Higgs and Z boson decays, respectively, while in the Upsilon(1S, 2S, 3S)gamma. final states the limits are (1.3, 1.9, 1.3) x 10(-3) and (3.4, 6.5, 5.4) x 10(-6), respectively. C1 [Jackson, P.; Lee, L.; Soni, N.; White, M. 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[Alexa, C.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Dobre, M.; Ducu, O. A.; Jinaru, A.; Maurer, J.; Olariu, A.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Horia Hulubei Natl Inst Phys & Nucl Engn, Bucharest 077125, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [y Garzon, G. Otero; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Robinson, D.; Thomson, M.; Ward, C. P.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Leight, W. A.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Abreu, R.; Aleksa, M.; Andari, N.; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boveia, A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Conti, G.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duehrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Perez, S. Fernandez; Francis, D.; Froidevaux, D.; Garonne, V.; Gianotti, F.; Gillberg, D.; Glatzer, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hawkings, R. J.; Heller, M.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Hubacek, Z.; Huhtinen, M.; Jaekel, M. R.; Jakobsen, S.; Jenni, P.; Kaneda, M.; Klioutchnikova, T.; Krasznahorkay, A.; Lantzsch, K.; Lapoire, C.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Marzin, A.; Messina, A.; Milic, A.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Rodrigues, L.; Roe, S.; Ruiz-Martinez, A.; Salzburger, A.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van Eldik, N.; van Woerden, M. C.; Vandelli, W.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Cheng, Y.; Dandoy, J. R.; Facini, G.; Fiascaris, M.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Krizka, K.; Li, H. L.; Melachrinos, C.; Merritt, F. S.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Vukotic, I.; Webster, J. S.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carquin, E.; Diaz, M. A.; Vogel, M.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Santiago, Chile. [Anulli, F.; Bai, Y.; Fang, Y.; Jin, S.; Lou, X.; Lu, F.; Ouyang, Q.; Ren, H.; Shan, L. Y.; Sun, X.; Wang, J.; Xu, D.; Yao, L.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guan, L.; Han, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, K.; Liu, M.; Liu, Y.; Peng, H.; Song, H. Y.; Xu, L.; Zhang, R.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Li, Y.; Wang, C.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Guo, J.; Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Dept Phys & Astron, Shanghai Key Lab Particle Phys & Cosmol, Shanghai 200030, Peoples R China. [Chen, X.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] CNRS, IN2P3, Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Cole, B.; Hu, D.; Hughes, E. W.; Klein, M. H.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Smith, M.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Aloisio, A.; Alonso, A.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Grp Coll Cosenza, Nazl Frascati Lab, Cosenza, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartmento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Camarda, S.; Deterre, C.; Filipuzzi, M.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yatsenko, E.; Yildirim, E.] DESY, Hamburg, Germany. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Camarda, S.; Deterre, C.; Filipuzzi, M.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yatsenko, E.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Erdmann, J.; Esch, H.; Gossling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Morgenstern, M.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, Sch Phys & Astron, SUPA, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Buescher, D.; Coniavitis, E.; Consorti, V.; Dao, V.; Di Simone, A.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Rave, T. C.; Ronzani, M.; Rosbach, K.; Ruhr, F.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; von Radziewski, H.; Warsinsky, M.; Weiser, C.; Werner, M.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Alexandre, G.; Ancu, L. S.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Bucci, F.; Toro, R. Camacho; Clark, A.; Delitzsch, C. M.; Della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Nessi, M.; Picazio, A.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, GE-380086 Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, D-35390 Giessen, Germany. [Bates, R. L.; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doherty, T.; Ferrag, S.; Ferrando, J.; De Lima, D. E. Ferreira; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; Morton, A.; Mullen, P.; O'Shea, V.; Barrera, C. Oropeza; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; Saxon, D. H.; Smith, K. M.; Denis, R. D. St.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, Sch Phys & Astron, SUPA, Glasgow, Lanark, Scotland. [Bindi, M.; Blumenschein, U.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Kareem, M. J.; Kawamura, G.; Keil, M.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Stolte, P.; Schroeder, T. Vazquez; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS, IN2P3, Labn Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Catastini, P.; Franklin, M.; Huth, J.; Ippolito, V.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Yen, A. L.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Dietzsch, T. A.; Djuvsland, J. I.; Dunford, M.; Hanke, P.; Jongmanns, J.; Khomich, A.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Heidelberg, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Castillo, L. R. Flores] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R. W.; Jussel, P.; Kneringer, E.; Lukas, W.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Krumnack, N.; Pluth, D.; Prell, S.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Kazarinov, M. Y.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Joint Nucl Res Inst, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Inamaru, Y.; Kishimoto, T.; Kurashige, H.; Kurumida, R.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Argentina. [Allison, L. J.; Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Readioff, N. P.; Schnellbach, Y. J.; Sultansoy, S.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Alpigiani, C.; Bevan, A. J.; Bona, M.; Bret, M. Cano; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, I.; Pilkington, A. D.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Jana, D. K.; Sawyer, L.; Sircar, A.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjoernmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Inst Fys, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Heck, T.; Hohlfeld, M.; Huesing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lin, T. H.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Poettgen, R.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schafer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Urrejola, P.; Wollstadt, S. J.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Keoshkerian, H.; Klinger, J. A.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Robinson, J. E. M.; Schwanenberger, C.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Liu, J.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Liu, J.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Jennens, D.; Kubota, T.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Hu, X.; Levin, D.; Liu, L.; Long, J. D.; Lu, N.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Panikashvili, N.; Qian, J.; Schwarz, T. A.; Searcy, J.; Thun, R. P.; Wilson, A.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Citterio, M.; Consonni, S. M.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazza, S. M.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Mazza, S. M.; Perini, L.; Pizio, C.; Ragusa, F.; Shojaii, S.; Simoniello, R.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Hrynevich, A.; Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Acad Sci, PN Lebedev Inst Phys, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Becker, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Elmsheuser, J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Schieck, J.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Benekos, N.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Manfredini, A.; Menke, S.; Moser, H. G.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Pahl, C.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Spettel, F.; Stern, S.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Conventi, F.; De Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Iengo, P.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Di Donato, C.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Klok, P. F.; Koenig, A. C.; Nektarijevic, S.; Salvucci, A.; Strubig, A.] Radboud Univ Nijmegen, Nikhef, Inst Math Astrophys & Particle Phys, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; De Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Keeler, R.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Adelman, J.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL USA. [Anisenkov, A. V.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Kharlamov, A.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; Van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, New York, NY 10003 USA. [Beacham, J. B.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; Gutierrez, P.; Hasib, A.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Bousson, N.; Haley, J.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.; Zhao, Y.] CNRS, IN2P3, F-91405 Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Read, A. L.; Rohne, O.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, K.; Beresford, L.; Boddy, C. R.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; King, R. S. B.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pachal, K.; Pickering, M. A.; Ryder, N. C.; Sawyer, C.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Kroll, J.; Lipeles, E.; Meyer, C.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Gonalo, R.; Jorge, P. M.; Lopes, L.; Machado Miguens, J.; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Galhardo, B.; Gomes, A.; Jorge, P. M.; Machado Miguens, J.; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Fac Ciencias & Tecnol, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, P.; Rybar, M.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] State Res Ctr Inst High Energy Phys, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Di Domenico, A.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Iuppa, R.; Liberti, B.; Mazzaferro, L.; Paolozzi, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Iuppa, R.; Mazzaferro, L.; Paolozzi, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Stanescu, C.; Taccini, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Taccini, C.; Trovatelli, M.] Univ Rome Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Techn Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA, Marrakech, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Cherkaoui El Moursli, R.; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mansoulie, B.; Martinez, H.; Meric, N.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.; Tsionou, D.] CEA Saclay Commissariat Energie Atom & Energ Alte, IRFU, DSM, Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grabas, H. M. X.; Grillo, A. A.; Kuhl, A.; Law, A. T.; Liang, Z.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Dawe, E.; Horton, A. J.; O'Neil, D. C.; Stelzer, B.; Tanasijczuk, A. J.; Torres, H.; van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Mount, R.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Strauss, E.; Su, D.; Swiatlowski, M.; Tompkins, L.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Federic, P.; Plazak, L.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnuclear Phys, Kosice 04353, Slovakia. [Hamilton, A.; Meehan, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Connell, S. H.; Lee, C. A.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Carrillo-Montoya, G. D.; Hamity, G. N.; Hsu, C.; March, L.; Garcia, B. R. Mellado; Ruan, X.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Eriksson, D.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Petridis, A.; Plucinski, P.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.] Stockholm Univ, Dept Phys, Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Rossetti, V.; Shcherbakova, A.; Sjolin, J.; Strandberg, S.; Tylmad, M.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys, Stony Brook, NY 11794 USA. [Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Chu, M. L.; Hou, S.; Hsu, P. J.; Jamin, D. O.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, S. M.; Yang, Y.; Zhang, L.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Guttman, N.; Munwes, Y.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgiou, K.; Hernandez, D. Paredes; Petridou, C.; Sampsonidis, D.; Sotiropoulou, C. L.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Aloisio, A.; Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Nobe, T.; Pettersson, N. E.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Diamond, M.; Ilic, N.; Krieger, P.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Schramm, S.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Gingrich, D. M.; Koutsman, A.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schneider, B.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.; Qureshi, A.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Moreno, D.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Barisonzi, M.; Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Quayle, W. B.; Shaw, K.; Soualah, R.] Ist Nazl Fis Nucl, Grp Collegato Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; Barisonzi, M.; Quayle, W. B.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Cavaliere, V.; Chang, P.; Errede, S.; Lie, K.; Liss, T. M.; Neubauer, M. S.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Kuutmann, E. Bergeaas; Brenner, R.; Buszello, C. P.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Urban, S. Cabrera; Castillo Gimenez, V.; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; De la Hoz, S. Gonzlez; Jimenez, Y. Hernandez; Hoign-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Urban, S. Cabrera; Castillo Gimenez, V.; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; De la Hoz, S. Gonzlez; Jimenez, Y. Hernandez; Hoign-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Urban, S. Cabrera; Castillo Gimenez, V.; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; De la Hoz, S. Gonzlez; Jimenez, Y. Hernandez; Hoign-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Urban, S. Cabrera; Castillo Gimenez, V.; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; De la Hoz, S. Gonzlez; Jimenez, Y. Hernandez; Hoign-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Inst Microelect Barcelona CNM, Valencia, Spain. [Urban, S. Cabrera; Castillo Gimenez, V.; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; De la Hoz, S. Gonzlez; Jimenez, Y. Hernandez; Hoign-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] CSIC, Valencia, Spain. [Danninger, M.; Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Swedish, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Berghaus, F.; David, C.; Elliot, A. A.; Fincke-Keeler, M.; Hamano, K.; Hill, E.; Kowalewski, R.; Kwan, T.; Lefebvre, M.; Marino, C. P.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.; Venturi, M.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Beckingham, M.; Farrington, S. M.; Harrison, P. F.; Janus, M.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Barak, L.; Bressler, S.; Citron, Z. H.; Duchovni, E.; Gross, E.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Pitt, M.; Roth, I.; Schaarschmidt, J.; Smakhtin, V.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Hard, A. S.; Heng, Y.; Ji, H.; Ju, X.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Kuger, F.; Redelbach, A.; Schreyer, M.; Sidiropoulou, O.; Siragusa, G.; Strohmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Julius Maximilians Univ, Fak Phys & Astron, Wurzburg, Germany. [Bannoura, A. A. E.; Beermann, T. A.; Braun, H. M.; Cornelissen, T.; Duda, D.; Ernis, G.; Fischer, J.; Fleischmann, S.; Flick, T.; Gabizon, O.; Hamacher, K.; Harenberg, T.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Kohlmann, S.; Lenzen, G.; Maettig, P.; Neumann, M.; Pataraia, S.; Riegel, C. J.; Sandhoff, M.; Tepel, F.; Wagner, W.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich C Phys, Wuppertal, Germany. [Baker, O. K.; Cummings, J.; Demers, S.; Garberson, F.; Guest, D.; Guillemin, T.; Henrichs, A.; Ideal, E.; Lagouri, T.; Leister, A. G.; Loginov, A.; Tipton, P.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] Ctr Calcul Inst Natl Phys Nucl & Phys Particules, IN2P3, Villeurbanne, France. [Acharya, B. S.] Kings Coll London, Dept Phys, London, England. Azerbaijan Acad Sci, Inst Phys, Baku 370143, Azerbaijan. [Anisenkov, A. V.; Bobrovnikov, V. S.; Korol, A. A.; Maslennikov, A. L.; Maximov, D. A.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Bawa, H. S.; Gao, Y. S.] Calif State Univ Fresno, Dept Phys, Fresno, CA USA. [Beck, H. P.] Univ Fribourg, Dept Phys, CH-1700 Fribourg, Switzerland. [Chelkov, G. A.] Tomsk State Univ, Tomsk 634050, Russia. [Conventi, F.; Davies, E.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Corriveau, F.; McPherson, R. A.; Robertson, S. H.; Sobie, R.; Teuscher, R. J.] Inst Particle Phys, Waterloo, ON, Canada. Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Fedin, O. L.] St Petersburg State Polytech Univ, Dept Phys, St Petersburg, Russia. [Greenwood, Z. D.; Sawyer, L.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Grinstein, S.; Rozas, A. Juste; Martinez, M.] ICREA, Barcelona, Spain. [Hsu, P. J.] Natl Tsing Hua Univ, Dept Phys, Hsinchu, Taiwan. [Ilchenko, Y.; Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Jejelava, J.] Ilia State Univ, Inst Theoret Phys, Tbilisi, Rep of Georgia. [Khubua, J.] Georgian Tech Univ, Tbilisi, Rep of Georgia. [Kono, T.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo 112, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Li, B.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei 115, Taiwan. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Pinamonti, M.] SISSA, Int Sch Adv Studies, I-34014 Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Shi, L.; Soh, D. A.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Tikhomirov, V. O.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Tompkins, L.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Vickey, T.] Univ Oxford, Dept Phys, Oxford, England. [Xu, L.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur, Malaysia. RP Yu, J (reprint author), Aix Marseille Univ, CPPM, Marseille, France. RI Gauzzi, Paolo/D-2615-2009; Mindur, Bartosz/A-2253-2017; Fabbri, Laura/H-3442-2012; Gutierrez, Phillip/C-1161-2011; Gerbaudo, Davide/J-4536-2012; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Peleganchuk, Sergey/J-6722-2014; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Olshevskiy, Alexander/I-1580-2016; Snesarev, Andrey/H-5090-2013; Ventura, Andrea/A-9544-2015; Kantserov, Vadim/M-9761-2015; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; KHODINOV, ALEKSANDR/D-6269-2015; Staroba, Pavel/G-8850-2014; Gladilin, Leonid/B-5226-2011; De, Kaushik/N-1953-2013; Carvalho, Joao/M-4060-2013; Mashinistov, Ruslan/M-8356-2015; Buttar, Craig/D-3706-2011; Smirnova, Oxana/A-4401-2013; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; Ferrando, James/A-9192-2012; Ciubancan, Liviu Mihai/L-2412-2015; Zhukov, Konstantin/M-6027-2015; Shmeleva, Alevtina/M-6199-2015; Gavrilenko, Igor/M-8260-2015; Veneziano, Stefano/J-1610-2012; Tikhomirov, Vladimir/M-6194-2015; Yang, Haijun/O-1055-2015; Chekulaev, Sergey/O-1145-2015; Warburton, Andreas/N-8028-2013; Gorelov, Igor/J-9010-2015; Riu, Imma/L-7385-2014; Costa, Maria Jose/H-5962-2015; Cavalli-Sforza, Matteo/H-7102-2015; Marti-Garcia, Salvador/F-3085-2011; Cortes Gonzalez, Arely/I-1034-2015; Della Pietra, Massimo/J-5008-2012; Petrucci, Fabrizio/G-8348-2012; Negrini, Matteo/C-8906-2014; Ferrer, Antonio/H-2942-2015; Grancagnolo, Sergio/J-3957-2015; Doyle, Anthony/C-5889-2009; spagnolo, stefania/A-6359-2012; Tassi, Enrico/K-3958-2015; Carquin, Edson/G-5221-2015; White, Ryan/E-2979-2015; Mir, Lluisa-Maria/G-7212-2015; Joergensen, Morten/E-6847-2015; Villa, Mauro/C-9883-2009; Livan, Michele/D-7531-2012; Brooks, William/C-8636-2013; Di Domenico, Antonio/G-6301-2011; Connell, Simon/F-2962-2015; Bosman, Martine/J-9917-2014; Boyko, Igor/J-3659-2013; Mitsou, Vasiliki/D-1967-2009 OI Gauzzi, Paolo/0000-0003-4841-5822; Mindur, Bartosz/0000-0002-5511-2611; Fabbri, Laura/0000-0002-4002-8353; Gerbaudo, Davide/0000-0002-4463-0878; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; SULIN, VLADIMIR/0000-0003-3943-2495; Vykydal, Zdenek/0000-0003-2329-0672; Olshevskiy, Alexander/0000-0002-8902-1793; Ventura, Andrea/0000-0002-3368-3413; Kantserov, Vadim/0000-0001-8255-416X; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Gladilin, Leonid/0000-0001-9422-8636; De, Kaushik/0000-0002-5647-4489; Carvalho, Joao/0000-0002-3015-7821; Mashinistov, Ruslan/0000-0001-7925-4676; Smirnova, Oxana/0000-0003-2517-531X; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; Ferrando, James/0000-0002-1007-7816; Ciubancan, Liviu Mihai/0000-0003-1837-2841; Veneziano, Stefano/0000-0002-2598-2659; Tikhomirov, Vladimir/0000-0002-9634-0581; Warburton, Andreas/0000-0002-2298-7315; Gorelov, Igor/0000-0001-5570-0133; Riu, Imma/0000-0002-3742-4582; Della Pietra, Massimo/0000-0003-4446-3368; Petrucci, Fabrizio/0000-0002-5278-2206; Negrini, Matteo/0000-0003-0101-6963; Ferrer, Antonio/0000-0003-0532-711X; Grancagnolo, Sergio/0000-0001-8490-8304; Doyle, Anthony/0000-0001-6322-6195; spagnolo, stefania/0000-0001-7482-6348; Carquin, Edson/0000-0002-7863-1166; White, Ryan/0000-0003-3589-5900; Mir, Lluisa-Maria/0000-0002-4276-715X; Joergensen, Morten/0000-0002-6790-9361; Villa, Mauro/0000-0002-9181-8048; Livan, Michele/0000-0002-5877-0062; Brooks, William/0000-0001-6161-3570; Di Domenico, Antonio/0000-0001-8078-2759; Connell, Simon/0000-0001-6000-7245; Bosman, Martine/0000-0002-7290-643X; Boyko, Igor/0000-0002-3355-4662; Mitsou, Vasiliki/0000-0002-1533-8886 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; ISF, MINERVA, GIF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 50 TC 10 Z9 10 U1 11 U2 56 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 26 PY 2015 VL 114 IS 12 AR 121801 DI 10.1103/PhysRevLett.114.121801 PG 19 WC Physics, Multidisciplinary SC Physics GA CE8EM UT WOS:000352074300004 ER PT J AU Schwessinger, B Bart, R Krasileva, KV Coaker, G AF Schwessinger, Benjamin Bart, Rebecca Krasileva, Ksenia V. Coaker, Gitta TI Focus issue on plant immunity: from model systems to crop species SO FRONTIERS IN PLANT SCIENCE LA English DT Editorial Material DE crops; agricultural; innate immunity; plant pathology; translational research; immune signaling ID RESISTANCE; PATHOGENS; WHEAT C1 [Schwessinger, Benjamin; Coaker, Gitta] Univ Calif Davis, Dept Plant Pathol, Davis, CA 95616 USA. [Schwessinger, Benjamin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint BioEnergy Inst, Berkeley, CA 94720 USA. [Schwessinger, Benjamin] Phys Biosci Div, Berkeley, CA 94720 USA. [Bart, Rebecca] Donald Danforth Plant Sci Ctr, St Louis, MO USA. [Krasileva, Ksenia V.] Norwich Res Pk, Genome Anal Ctr, Norwich, Norfolk, England. [Krasileva, Ksenia V.] Norwich Res Pk, Sainsbury Lab, Norwich, Norfolk, England. RP Schwessinger, B (reprint author), Univ Calif Davis, Dept Plant Pathol, Davis, CA 95616 USA. EM bschwessinger@ucdavis.edu; glcoaker@ucdavis.edu RI Bart, Rebecca/M-2838-2013; OI Schwessinger, Benjamin/0000-0002-7194-2922; Bart, Rebecca/0000-0003-1378-3481 FU NIGMS NIH HHS [R01 GM092772] NR 24 TC 3 Z9 3 U1 2 U2 19 PU FRONTIERS RESEARCH FOUNDATION PI LAUSANNE PA PO BOX 110, LAUSANNE, 1015, SWITZERLAND SN 1664-462X J9 FRONT PLANT SCI JI Front. Plant Sci. PD MAR 26 PY 2015 VL 6 AR 195 DI 10.3389/fpls.2015.00195 PG 3 WC Plant Sciences SC Plant Sciences GA CF4EX UT WOS:000352502600001 PM 25859255 ER PT J AU Goldstein, S Behar, D Rajh, T Rabani, J AF Goldstein, Sara Behar, David Rajh, Tijana Rabani, Joseph TI Nitric Oxide Reduction to Ammonia by TiO2 Electrons in Colloid Solution via Consecutive One-Electron Transfer Steps SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID SELECTIVE PHOTOCATALYTIC REDUCTION; TRANSIENT ABSORPTION-SPECTROSCOPY; CONDUCTION-BAND ELECTRONS; AQUEOUS-SOLUTIONS; OPTICAL ELECTROCHEMISTRY; SEMICONDUCTOR ELECTRODE; PULSE-RADIOLYSIS; CHARGE-TRANSFER; DYNAMICS; NANOPARTICLES AB The reaction mechanism of nitric oxide (NO) reduction by excess electrons on TiO2 nanoparticles (e(TiO2)-) has been studied under anaerobic conditions. TiO2 was loaded with 10-130 electrons per particle using gamma-irradiation of acidic TiO2 colloid solutions containing 2-propanol. The study is based on time-resolved kinetics and reactants and products analysis. The reduction of NO by e(TiO2)- is interpreted in terms of competition between a reaction path leading to formation of NH3 and a path leading to N2O and N-2. The proposed mechanism involves consecutive one-electron transfers of NO, and its reduction intermediates HNO, NH2O, and NH2OH. The results show that e(TiO2)- does not reduce N2O and N-2. Second-order rate constants of e(TiO2)- reactions with NO (740 +/- 30 M-(1) s-(1)) and NH2OH (270 +/- 30 M-(1) s-(1)) have been determined employing the rapid-mixing stopped-flow technique and that with HNO (>1.3 x 106 M-(1) s-(1)) was derived from fitting the kinetic traces to the suggested reaction mechanism, which is discussed in detail. C1 [Goldstein, Sara; Behar, David; Rabani, Joseph] Hebrew Univ Jerusalem, Inst Chem, IL-91904 Jerusalem, Israel. [Goldstein, Sara; Behar, David; Rabani, Joseph] Hebrew Univ Jerusalem, Accelerator Lab, IL-91904 Jerusalem, Israel. [Rajh, Tijana] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. RP Rabani, J (reprint author), Hebrew Univ Jerusalem, Inst Chem, IL-91904 Jerusalem, Israel. EM rabani@mail.huji.ac.il FU US-Israel BSF [2012158] FX This work was generously supported by the US-Israel BSF under Contract no. 2012158. We acknowledge with thanks the invaluable assistance by Dr. Inna Popov from the Center for Nanoscience and Nanotechnology, at the Hebrew University of Jerusalem. NR 40 TC 5 Z9 5 U1 8 U2 35 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD MAR 26 PY 2015 VL 119 IS 12 BP 2760 EP 2769 DI 10.1021/jp5102863 PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CE6TP UT WOS:000351971400003 PM 25730520 ER PT J AU Jackson, VE Felmy, AR Dixon, DA AF Jackson, Virgil E. Felmy, Andrew R. Dixon, David A. TI Prediction of the pK(a)'s of Aqueous Metal Ion+2 Complexes SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID X-RAY-DIFFRACTION; MOLECULAR-DYNAMICS SIMULATION; HYDRATION SHELL STRUCTURE; DENSITY-FUNCTIONAL THEORY; COUPLED-CLUSTER THEORY; CONSISTENT BASIS-SETS; CONVERGENT BASIS-SETS; CRYSTAL-STRUCTURE; CALCIUM-ION; FREE-ENERGY AB Aqueous metal ions play an important role in many areas of chemistry. The acidities of [Be(H2O)(4)](2+), [M(H2O)(6)](2+), M = Mg2+, Mn2+, Fe2+, Co2+, Ni2+, Cu2+, Zn2+, Cd2+, and Hg2+, and [M(H2O)n](2+), M = Ca2+ and Sr2+, n = 7 and 8, complexes have been predicted using density functional theory, second-order Moller-Plesset perturbation theory (MP2), and coupled cluster CCSD(T) theory in the gas phase. pK(a)'s in aqueous solution were predicted by using self-consistent reaction field (SCRF) calculations with different solvation models. The most common binding motif of the majority of the metal +2 complexes is coordination number (CN) 6, with each hexaaquo cluster having reasonably high symmetry for the best arrangement of the water molecules in the first solvation shell. Be2+ is tetracoordinated, but a second solvation shell of 8 waters is needed to predict the pK(a). The Ca2+ and Sr2+ aquo clusters have a coordination number of 7 or 8 as found in terms of the energy of the reaction M(H2O)(7)(2+) + (HO)-O-2 -> M(H2O)(8)(2+) and the pK(a) values. The calculated geometries are in reasonable agreement with experiment. The SCRF calculations with the conductor-like screening model (COSMO), and the conductor polarized continuum model (CPCM) using COSMO-RS radii, consistently agree best with experiment at the MP2/aug-cc-pVDZ and CCSD(T)/aug-cc-pVDZ levels of theory. The CCSD(T) level provides the most accurate pK(a)'s, and the MP2 level also provides reliable predictions. Our predictions were used to elucidate the properties of metal +2 ion complexes. The pK(a) predictions provide confirmation of the size of the first solvation shell sizes. The calculations show that it is still difficult to predict pK(a)'s using this cluster/implicit solvent approach to better than 1 pK(a) unit. C1 [Jackson, Virgil E.; Dixon, David A.] Univ Alabama, Dept Chem, Tuscaloosa, AL 35487 USA. [Felmy, Andrew R.] Pacific NW Natl Lab, Fundamental Sci Directorate, Richland, WA 99352 USA. RP Dixon, DA (reprint author), Univ Alabama, Dept Chem, Shelby Hall, Tuscaloosa, AL 35487 USA. EM dadixon@bama.ua.edu FU U.S. Department of Energy (DOE), Office of Basic Energy Sciences Geosciences program [DE-SC0009362]; Robert Ramsay Chair Fund of The University of Alabama FX This work was supported by the U.S. Department of Energy (DOE), Office of Basic Energy Sciences Geosciences program grant number DE-SC0009362. DAD. thanks the Robert Ramsay Chair Fund of The University of Alabama for support. NR 98 TC 3 Z9 3 U1 4 U2 39 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD MAR 26 PY 2015 VL 119 IS 12 BP 2926 EP 2939 DI 10.1021/jp5118272 PG 14 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CE6TP UT WOS:000351971400021 PM 25721568 ER PT J AU Wu, H Tang, WS Stavila, V Zhou, W Rush, JJ Udovic, TJ AF Wu, Hui Tang, Wan Si Stavila, Vitalie Zhou, Wei Rush, John J. Udovic, Terrence J. TI Structural Behavior of Li2B10H10 SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID CRYSTAL-STRUCTURES; LI2B12H12; DECOMPOSITION; STABILITY; NA; VISUALIZATION; CA(BH4)(2); TRANSITION; DESORPTION; SCATTERING AB On the basis of ray and neutron powder diffraction, fit-principles calculations, and neutron vibrational spectroscopy, Li2B10H10 was found to exhibit atypical hexagonal symmetry to best stabilize the ionic packing of the relatively small Li cations and largeiellipsoidal B10H102- anions. Moreover, differential scanning calarimetry and neutron-elastic-scattering fixed-window scans suggested that Li2B10H10, similar to its polyhedral cousin Li2B12H12, undergoes an order-disorder phase transition near 640 K. These results provide valuable structural information pertinent to understanding the potential role that L4B10H10 plays during LiBH4 dehydrogenation-rehydrogenation as well as its prospects as a superionic Li+ cation conductor. C1 [Wu, Hui; Tang, Wan Si; Zhou, Wei; Rush, John J.; Udovic, Terrence J.] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Wu, Hui; Tang, Wan Si; Zhou, Wei; Rush, John J.] Univ Maryland, Dept Mat Sci & Engn, College Pk, MD 20742 USA. [Stavila, Vitalie] Sandia Natl Labs, Energy Nanomat, Livermore, CA 94551 USA. RP Wu, H (reprint author), NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. EM hui.wu@nist.gov; udovic@nist.gov RI Wu, Hui/C-6505-2008; Zhou, Wei/C-6504-2008 OI Wu, Hui/0000-0003-0296-5204; Zhou, Wei/0000-0002-5461-3617 FU DOE EERE [DE-EE0002978]; National Science Foundation [DMR-0944772] FX This work was partially supported by the DOE EERE under Grant No. DE-EE0002978 and utilized facilities supported in part by the National Science Foundation under Agreement DMR-0944772. NR 39 TC 11 Z9 11 U1 1 U2 25 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAR 26 PY 2015 VL 119 IS 12 BP 6481 EP 6487 DI 10.1021/acs.jpcc.5b00533 PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CE6TJ UT WOS:000351970800004 ER PT J AU Parkes, MV Sava Gallis, DF Greathouse, JA Nenoff, TM AF Parkes, Marie V. Sava Gallis, Dorina F. Greathouse, Jeffery A. Nenoff, Tina M. TI Effect of Metal in M-3(btc)(2) and M-2(dobdc) MOFs for O-2/N-2 Separations: A Combined Density Functional Theory and Experimental Study SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID ORGANIC FRAMEWORK MATERIALS; CAMBRIDGE STRUCTURAL DATABASE; IRON(II) COORDINATION SITES; AUGMENTED-WAVE METHOD; GAS-ADSORPTION; MOLECULAR-SIEVE; AIR SEPARATION; HYDROGEN ADSORPTION; CRYSTAL-STRUCTURES; ROOM-TEMPERATURE AB Computational screening of metal-organic framework (MOF) materials for selective oxygen adsorption from air is used to identify new sorbents for oxyfuel combustion process feedstock-streams. A comprehensive study on the effect of MOF metal chemistry on,gas binding energies in two common but structurally disparate MOFs has been undertaken. Dispersion-corrected,density functional theory (DFT) methods were used to calculate the oxygen and nitrogen binding energies with each of 14 metals, respectively, substituted into two MOF series, M-2(dobdc) and M-3(btc)(2). The accuracy of DFT methods was validated by comparing trends in binding energy with experimental gas sorption measurements A periodic trend in oxygen binding energies was found, with greater oxygen binding energies for early transition-metal-substituted MOFS compared to late transition metal MOFS; this was independent of MOF Structural type. The larger binding energies were associated with oxygen binding in a side-on Configuration to the metal, with concomitant lengthening of the O-O bond In contrast, nitrogen binding energies Were similar across the transition metal series, regardless of both MOF structural type and metal identity. Taken together, these findings suggest that early transition metal MOFs are best suited to separating oxygen from, nitrogen and that the MOF structural type is legs important than the metal identity. C1 [Parkes, Marie V.; Greathouse, Jeffery A.] Sandia Natl Labs, Geochem Dept, Albuquerque, NM 87185 USA. [Sava Gallis, Dorina F.; Nenoff, Tina M.] Sandia Natl Labs, Nanoscale Sci Dept, Albuquerque, NM 87185 USA. RP Greathouse, JA (reprint author), Sandia Natl Labs, Geochem Dept, POB 5800, Albuquerque, NM 87185 USA. EM jagreat@sandia.gov; tmnenof@sandia.gov RI Sava Gallis, Dorina/D-2827-2015 FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; Sandia's Laboratory Directed Research and Development program FX Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL85000. This research was funded by Sandia's Laboratory Directed Research and Development program. NR 86 TC 8 Z9 8 U1 4 U2 52 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAR 26 PY 2015 VL 119 IS 12 BP 6556 EP 6567 DI 10.1021/jp511789g PG 12 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CE6TJ UT WOS:000351970800012 ER PT J AU Majola, SNT Hartley, DJ Riedinger, LL Sharpey-Schafer, JF Allmond, JM Beausang, C Carpenter, MP Chiara, CJ Cooper, N Curien, D Gall, BJP Garrett, PE Janssens, RVF Kondev, FG Kulp, WD Lauritsen, T McCutchan, EA Miller, D Piot, J Redon, N Riley, MA Simpson, J Stefanescu, I Werner, V Wang, X Wood, JL Yu, CH Zhu, S AF Majola, S. N. T. Hartley, D. J. Riedinger, L. L. Sharpey-Schafer, J. F. Allmond, J. M. Beausang, C. Carpenter, M. P. Chiara, C. J. Cooper, N. Curien, D. Gall, B. J. P. Garrett, P. E. Janssens, R. V. F. Kondev, F. G. Kulp, W. D. Lauritsen, T. McCutchan, E. A. Miller, D. Piot, J. Redon, N. Riley, M. A. Simpson, J. Stefanescu, I. Werner, V. Wang, X. Wood, J. L. Yu, C. -H. Zhu, S. TI Observation of gamma vibrations and alignments built on non-ground-state configurations in Dy-156 SO PHYSICAL REVIEW C LA English DT Article ID BAND-CROSSING FREQUENCIES; PROJECTED SHELL-MODEL; HIGH-SPIN; ROTATIONAL BANDS; DEFORMED-NUCLEI; QUASI-PARTICLE; REGION; ER-164; GD-154; SPECTROSCOPY AB The exact nature of the lowest K-pi = 2(+) rotational bands in all deformed nuclei remains obscure. Traditionally they are assumed to be collective vibrations of the nuclear shape in the. degree of freedom perpendicular to the nuclear symmetry axis. Very few such. bands have been traced past the usual backbending rotational alignments of high-j nucleons. We have investigated the structure of positive-parity bands in the N = 90 nucleus Dy-156, using the Nd-148(C-12,4n) Dy-156 reaction at 65 MeV, observing the resulting. gamma-ray transitions with the Gammasphere array. The even-and odd-spin members of the K-pi = 2(+)gamma band are observed up to 32(+) and 31(+), respectively. This rotational band faithfully tracks the ground-state configuration to the highest spins. The members of a possible. vibration built on the aligned yrast S band are observed up to spins 28(+) and 27(+). An even-spin positive-parity band, observed up to spin 24(+), is a candidate for an aligned S band built on the seniority-zero configuration of the 0(2)(+) state at 676 keV. The crossing of this band with the 0(2)(+) band is at h omega(c) = 0.28(1) MeV and is consistent with the configuration of the 0(2)(+) band not producing any blocking of the monopole pairing. C1 [Majola, S. N. T.] Natl Res Fdn, iThemba LABS, ZA-7129 Somerset West, South Africa. [Majola, S. N. T.] Univ Cape Town, Dept Phys, ZA-7701 Rondebosch, South Africa. [Hartley, D. J.] US Naval Acad, Dept Phys, Annapolis, MD 21402 USA. [Riedinger, L. L.; Miller, D.] Univ Tennessee, Dept Phys, Knoxville, TN 37996 USA. [Sharpey-Schafer, J. F.] Univ Western Cape, Dept Phys, ZA-7535 Bellville, South Africa. [Allmond, J. M.; Beausang, C.] Univ Richmond, Dept Phys, Richmond, VA 23173 USA. [Carpenter, M. P.; Janssens, R. V. F.; Lauritsen, T.; McCutchan, E. A.; Stefanescu, I.; Zhu, S.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Chiara, C. J.; Kondev, F. G.] Argonne Natl Lab, Nucl Engn Div, Argonne, IL 60439 USA. [Cooper, N.; Werner, V.] Yale Univ, Wright Nucl Struct Lab, New Haven, CT 06520 USA. [Curien, D.; Gall, B. J. P.; Piot, J.] Univ Strasbourg, IPHC, F-67037 Strasbourg, France. [Curien, D.; Gall, B. J. P.; Piot, J.] CNRS, UMR7178, F-67037 Strasbourg, France. [Garrett, P. E.] Univ Guelph, Dept Phys, Guelph, ON N1G 2W1, Canada. [Kulp, W. D.; Wood, J. L.] Georgia Inst Technol, Sch Phys, Atlanta, GA 30332 USA. [McCutchan, E. A.] Brookhaven Natl Lab, Natl Nucl Data Ctr, Upton, NY 11973 USA. [Redon, N.] CNRS, IN2P3, Inst Phys Nucl Lyon, F-69622 Villeurbanne, France. [Riley, M. A.; Wang, X.] Florida State Univ, Dept Phys, Tallahassee, FL 32306 USA. [Simpson, J.] STFC, Daresbury Lab, Warrington WA4 4AD, Cheshire, England. [Allmond, J. M.; Yu, C. -H.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. RP Majola, SNT (reprint author), Natl Res Fdn, iThemba LABS, POB 722, ZA-7129 Somerset West, South Africa. EM majola@tlabs.ac.za RI Carpenter, Michael/E-4287-2015; Miller, David/B-5372-2012; Werner, Volker/C-1181-2017 OI Carpenter, Michael/0000-0002-3237-5734; Miller, David/0000-0002-0426-974X; Werner, Volker/0000-0003-4001-0150 FU U.S. National Science Foundation [PHY-1203100, PHY-0754674]; U.S. Department of Energy, Office of Nuclear of Nuclear Physics [DE-AC02-06CH11357, DE-FG02-91ER40609]; Joyce Frances Adlard Cultural Fund; South African National Research Foundation FX We would like to thank the crew of the ANL ATLAS accelerator for delivering a very stable and clean beam. The authors also thank the ANL operations staff at Gammasphere and gratefully acknowledge the efforts of J. P. Green for target preparation. In addition we thank D. Radford for software support and S. Aberg for constructive discussions. This work was funded by the U.S. National Science Foundation under Grants No. PHY-1203100 (USNA) and No. PHY-0754674 (FSU) as well as by the U.S. Department of Energy, Office of Nuclear of Nuclear Physics, under Contracts No. DE-AC02-06CH11357 (ANL) and No. DE-FG02-91ER40609 (Yale). One of us J.F.S.-S. would like to thank the Joyce Frances Adlard Cultural Fund for support. S.N.T.M. acknowledges a postgraduate grant from the South African National Research Foundation and thanks the library staff of iThemba LABS for considerable help. NR 59 TC 3 Z9 3 U1 1 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAR 26 PY 2015 VL 91 IS 3 AR 034330 DI 10.1103/PhysRevC.91.034330 PG 9 WC Physics, Nuclear SC Physics GA CE7LR UT WOS:000352022400002 ER PT J AU Bonamici, CE Fanning, CM Kozdon, R Fournelle, JH Valley, JW AF Bonamici, Chloe E. Fanning, C. Mark Kozdon, Reinhard Fournelle, John H. Valley, John W. TI Combined oxygen-isotope and U-Pb zoning studies of titanite: New criteria for age preservation SO CHEMICAL GEOLOGY LA English DT Article DE Titanite; U-Pb dating; Oxygen isotopes; SIMS; Zoning; Diffusion; Adirondack Mountains ID COLTON MYLONITE ZONE; T-T PATH; NEW-YORK; ADIRONDACK MOUNTAINS; GRENVILLE PROVINCE; CLOSURE TEMPERATURE; CRYSTAL-CHEMISTRY; OROGENIC COLLAPSE; ION MICROPROBE; COOLING RATES AB Titanite is an important U-Pb chronometer for dating geologic events, but its high-temperature applicability depends upon its retention of radiogenic lead (Pb). Experimental data predict similar rates of diffusion for lead (Pb) and oxygen (O) in titanite at granulite-facies metamorphic conditions (T = 650-800 degrees C). This study therefore investigates the utility of O-isotope zoning as an indicator for U-Pb zoning in natural titanite samples from the Carthage-Colton Mylonite Zone of the Adirondack Mountains, New York. Based on previous field, textural, and microanalytical work, there are four generations (types) of titanite in the study area, at least two of which preserve diffusion-related delta O-18 zoning. U-Th-Pb was analyzed by SIMS along traverses across three grains of type-2 titanite, which show well-developed diffusional delta O-18 zoning, and one representative grain from each of the other titanite generations. Type-2 and type-4 titanites show broadly core-to-rim decreasing Pb-206/U-238 zoning, consistent with Pb diffusion at higher temperatures, and uniform or even slightly increasing Pb-206/U-238 near grain rims, indicating subsequent recrystallization and/or new growth below the Pb blocking temperature. Type-2 and type-4 grain cores preserve ca. 1160 Ma ages that correlate with the anorthosite-mangerite-charnockite-granite magmatic phase of the Grenville orogeny, whereas grain rims give ca. 1050 Ma Pb-206/U-238 ages that coincide with the culminating Ottawan phase. The type-3 titanite grain was sampled from a vein and yields Pb-206/U-238 dates older than the syenite into which the vein was emplaced; accordingly, its Pb-206/U-238 dates are interpreted as indicating excess uncorrected common Pb. Type-2 grains with recrystallized or shear-eroded margins show truncated or reversed Pb-206/U-238 zoning but retain symmetrically decreasing delta O-18 zoning, consistent with grain margin modification following arrest of Pb diffusion but before arrest of O diffusion. It is concluded that O diffusion was slightly faster than Pb diffusion in Adirondack titanites at the conditions of (local) peak Ottawan metamorphism, making delta O-18 zoning a useful discriminator of closed-system age domains that did not suffer Pb loss. In addition, the small offset in the O and Pb partial retention zones constrains the timing and temperature of oblique-slip deformation along the Carthage-Colton Mylonite Zone: the details of porphyroclast microstructure and zoning data show that the oblique-slip shear zones were active at ca. 1050 Ma, with deformation initiating near the peak of Ottawan metamorphism at similar to 700 degrees C and continuing through the O blocking temperature at similar to 550 degrees C. Published by Elsevier B.V. C1 [Bonamici, Chloe E.; Kozdon, Reinhard; Fournelle, John H.; Valley, John W.] Univ Wisconsin, WiscSIMS, Dept Geosci, Madison, WI 53706 USA. [Bonamici, Chloe E.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Fanning, C. Mark] Australian Natl Univ, Res Sch Earth Sci, Canberra, ACT 0200, Australia. RP Bonamici, CE (reprint author), Los Alamos Natl Lab, POB 1663,MS j514, Los Alamos, NM 87545 USA. RI Kozdon, Reinhard/J-9468-2014; Fanning, C. Mark/I-6449-2016 OI Kozdon, Reinhard/0000-0001-6347-456X; Fanning, C. Mark/0000-0003-3331-3145 FU U.S. National Science Foundation [EAR-0838058]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-FG02-93ER14389]; Geological Society of America student research grant [9224-10]; [NSF-EAR-1053466]; [1355590] FX We thank Noriko Kita, Kouki Kitajima, Ariel Strickland, and Jim Kern for assistance in the WiscSIMS lab and Brian Hess for sample preparation. We thank Dr. Xavier Llovet for instrument time at the University of Barcelona. Laurel Goodwin and Brad Singer provided helpful comments on this manuscript. John Craven and John Aleinikoff provided titanite standards. John Aleinikoff, Andrew Kylander-Clark, and an anonymous individual provided thorough, helpful reviews. This material is based upon work supported by the U.S. National Science Foundation (award EAR-0838058), the U.S. Department of Energy, Office of Basic Energy Sciences under Award Number DE-FG02-93ER14389, and Geological Society of America student research grant 9224-10. WiscSIMS is partially supported by NSF-EAR-1053466 and - 1355590. NR 57 TC 7 Z9 8 U1 4 U2 10 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2541 EI 1878-5999 J9 CHEM GEOL JI Chem. Geol. PD MAR 26 PY 2015 VL 398 BP 70 EP 84 DI 10.1016/j.chemgeo.2015.02.002 PG 15 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA CE2TV UT WOS:000351672600007 ER PT J AU Bierlich, C Gustafson, G Lonnblad, L Tarasov, A AF Bierlich, Christian Gustafson, Gosta Lonnblad, Leif Tarasov, Andrey TI Effects of overlapping strings in pp collisions SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE QCD Phenomenology; Monte Carlo Simulations ID HEAVY-ION COLLISIONS; NUCLEUS-NUCLEUS COLLISIONS; GLUON DISTRIBUTION-FUNCTIONS; CHROMOELECTRIC-FLUX-TUBE; DUAL PARTON MODEL; TO-LEADING BFKL; PAIR PRODUCTION; TRANSVERSE-MOMENTUM; PARTICLE-PRODUCTION; BARYON PRODUCTION AB In models for hadron collisions based on string hadronization, the strings are usually treated as independent, allowing no interaction between the confined colour fields. In studies of nucleus collisions it has been suggested that strings close in space can fuse to form "colour ropes". Such ropes are expected to give more strange particles and baryons, which also has been suggested as a signal for plasma formation. Overlapping strings can also be expected in pp collisions, where usually no phase transition is expected. In particular at the high LHC energies the expected density of strings is quite high. To investigate possible effects of rope formation, we present a model in which strings are allowed to combine into higher multiplets, giving rise to increased production of baryons and strangeness, or recombine into singlet structures and vanish. Also a crude model for strings recombining into junction structures is considered, again giving rise to increased baryon production. The models are implemented in the dipsy MC event generator, using Pythia8 for hadronization, and comparison to pp minimum bias data, reveals improvement in the description of identified particle spectra. C1 [Bierlich, Christian; Gustafson, Gosta; Lonnblad, Leif] Lund Univ, Dept Astron & Theoret Phys, Lund, Sweden. [Tarasov, Andrey] Jefferson Lab, Ctr Theory, Newport News, VA USA. RP Bierlich, C (reprint author), Lund Univ, Dept Astron & Theoret Phys, Solvegatan 14A, Lund, Sweden. EM christian.bierlich@thep.lu.se; gosta.gustafson@thep.lu.se; leif.lonnblad@thep.lu.se; atarasov@jlab.org FU MCnetITN FP7 Marie Curie Initial Training Network [PITN-GA-2012-315877]; Swedish Research Council [621-2012-2283, 621-2013-4287]; Jefferson Science Associates, LLC [DE-AC05-06OR23177] FX Work supported in part by the MCnetITN FP7 Marie Curie Initial Training Network, contract PITN-GA-2012-315877, the Swedish Research Council (contracts 621-2012-2283 and 621-2013-4287), and contract DE-AC05-06OR23177 under which the Jefferson Science Associates, LLC operates the Thomas Jefferson National Accelerator Facility. NR 94 TC 9 Z9 9 U1 0 U2 3 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAR 26 PY 2015 IS 3 AR 148 DI 10.1007/JHEP03(2015)148 PG 49 WC Physics, Particles & Fields SC Physics GA CE3TG UT WOS:000351751200008 ER PT J AU Lee, IH Saha, S Polley, A Huang, H Mayor, S Rao, M Groves, JT AF Lee, Il-Hyung Saha, Suvrajit Polley, Anirban Huang, Hector Mayor, Satyajit Rao, Madan Groves, Jay T. TI Live Cell Plasma Membranes Do Not Exhibit a Miscibility Phase Transition over a Wide Range of Temperatures SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID FLUORESCENCE CORRELATION SPECTROSCOPY; DYNAMIC LIGHT-SCATTERING; SINGLE-MOLECULE; LIPID RAFTS; CRITICAL FLUCTUATIONS; MODEL MEMBRANES; CORTICAL ACTIN; DIFFUSION LAWS; VESICLES; ORGANIZATION AB Lipid/cholesterol mixtures derived from cell membranes as well as their synthetic reconstitutions exhibit well-defined miscibility phase transitions and critical phenomena near physiological temperatures. This suggests that lipid/cholesterol-mediated phase separation plays a role in the organization of live cell membranes. However, macroscopic lipid phase separation is not generally observed in cell membranes, and the degree to which properties of isolated lipid mixtures are preserved in the cell membrane remain unknown. A fundamental property of phase transitions is that the variation of tagged particle diffusion with temperature exhibits an abrupt change as the system passes through the transition, even when the two phases are distributed in a nanometer-scale emulsion. We support this using a variety of Monte Carlo and atomistic simulations on model lipid membrane systems. However, temperature-dependent fluorescence correlation spectroscopy of labeled lipids and membrane-anchored proteins in live cell membranes shows a consistently smooth increase in the diffusion coefficient as a function of temperature. We find no evidence of a discrete miscibility phase transition throughout a wide range of temperatures: 14-37 degrees C. This contrasts the behavior of giant plasma membrane vesicles (GPMVs) blebbed from the same cells, which do exhibit phase transitions and macroscopic phase separation. Fluorescence lifetime analysis of a DiI probe in both cases reveals a significant environmental difference between the live cell and the GPMV. Taken together, these data suggest the live cell membrane may avoid the miscibility phase transition inherent to its lipid constituents by actively regulating physical parameters, such as tension, in the membrane. C1 [Lee, Il-Hyung; Huang, Hector; Groves, Jay T.] Univ Calif Berkeley, Dept Chem, Howard Hughes Med Inst, Calif Inst Quantitat Biosci QB3, Berkeley, CA 94720 USA. [Groves, Jay T.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Phys Biosci Div, Berkeley, CA 94720 USA. [Saha, Suvrajit; Mayor, Satyajit; Rao, Madan] Natl Ctr Biol Sci TIFR, Bangalore 560065, Karnataka, India. [Polley, Anirban; Rao, Madan] Raman Res Inst, Bangalore 560080, Karnataka, India. RP Groves, JT (reprint author), Univ Calif Berkeley, Dept Chem, Howard Hughes Med Inst, Calif Inst Quantitat Biosci QB3, Berkeley, CA 94720 USA. EM JTGroves@lbl.gov RI Rao, Madan/E-2927-2012; OI Saha, Suvrajit/0000-0001-6631-0464 FU Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX We acknowledge Prof. Adam Smith for help in experimental design and optical alignment. We also acknowledge Dr. Christopher Rhodes and Dr. Michael Coyle for FCS data analysis and Ann Fischer from UC Berkeley Tissue Culture Facility for mammalian cell cultures. We thank Prof. Sarah Veatch for kindly providing the data we used for Figure 7a ternary mixture phase diagram. This work was supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 69 TC 10 Z9 11 U1 5 U2 26 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAR 26 PY 2015 VL 119 IS 12 BP 4450 EP 4459 DI 10.1021/jp512839q PG 10 WC Chemistry, Physical SC Chemistry GA CE6TM UT WOS:000351971100011 PM 25747462 ER PT J AU Sharma, VK Mamontov, E Anunciado, DB O'Neill, H Urban, V AF Sharma, V. K. Mamontov, E. Anunciado, D. B. O'Neill, H. Urban, V. TI Nanoscopic Dynamics of Phospholipid in Unilamellar Vesicles: Effect of Gel to Fluid Phase Transition SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID ELASTIC NEUTRON-SCATTERING; LIPID-BILAYERS; LATERAL DIFFUSION; MOLECULAR-DYNAMICS; MEMBRANES; MICELLES; MODEL; SPECTROSCOPY; SIMULATIONS; INTERFACE AB The dynamics of phospholipids in unilamellar vesicles (ULVs) is of interest in biology, medical; and food sciences; since these molecules are widely used as biocompatible agents and a mimic of tell Membrane systems. We have investigated the nanoscopic dynamics of 1,2-dimyristoyl-sn-glycero-3-phosphocholine (DMPC) phospholipid in ULVs as a function of temperature using elastic and quasielastic neutron scattering (QENS). The dependence of the signal on the scattering momentum transfer, which is a critical advantage of neutron scattering techniques, allows the detailed analysis of the lipid motions that cannot be carried out by other means. In agreement with a differential scanning calorimetry measurement, a sharp rise in the elastic scattering intensity below ca. 296 K indicates a phase transition from the high-temperature fluid phase to the low-temperature solid gel phase. The microscopic lipid dynamics exhibits qualitative differences between the solid gel phase (in a measurement at 280 K) and the fluid phase (in a measurement at a physiological temperature of 310 K). The analysis of the data demonstrates the presence of two types of distinct motions: the entire lipid molecule motion within a monolayer, also known as lateral diffusion, and the relatively faster internal motion of the DMPC molecule. The lateral diffusion of the entire lipid molecule is Fickian in character, whereas the internal lipid motions are of localized character, which is consistent with the structure of the vesicles. The lateral motion slows down by an order of magnitude in the solid gel phase, whereas for the internal motion not only the time scale but also the character of the motion changes upon the phase transition. In the solid gel phase, the lipids are more ordered and undergo uniaxial rotational motion. However, in the fluid phase, the hydrogen atoms of the lipid tails undergo confined translation diffusion rather than uniaxial rotational diffusion. The translational, but spatially localized, diffusion of the hydrogen atoms of the lipid tails is a manifestation of the flexibility of the chains acquired in the fluid phase. Because of this flexibility, both the local diffusivity and the confinement volume for the hydrogen atoms increase in the linear fashion from near the lipid's polar headgroup to the end of its hydrophobic tail. Our results present a quantitative and detailed picture of the effect of the gel-fluid phase transition on the nanoscopic lipid dynamics in ULVs. The data analysis approach developed here has a potential for probing the dynamic response of lipids to the presence of additional cell membrane components. C1 [Sharma, V. K.; Anunciado, D. B.; O'Neill, H.; Urban, V.] Oak Ridge Natl Lab, Biol & Soft Matter Div, Neutron Sci Directorate, Oak Ridge, TN 37831 USA. [Sharma, V. K.] Bhabha Atom Res Ctr, Div Solid State Phys, Bombay 400085, Maharashtra, India. [Mamontov, E.] Oak Ridge Natl Lab, Chem & Engn Mat Div, Neutron Sci Directorate, Oak Ridge, TN 37831 USA. RP Sharma, VK (reprint author), Oak Ridge Natl Lab, Biol & Soft Matter Div, Neutron Sci Directorate, Oak Ridge, TN 37831 USA. EM sharmavk@ornl.gov RI Urban, Volker/N-5361-2015; Mamontov, Eugene/Q-1003-2015; OI Urban, Volker/0000-0002-7962-3408; Mamontov, Eugene/0000-0002-5684-2675; O'Neill, Hugh/0000-0003-2966-5527 FU Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy; Office of Biological and Environmental Research [ERKP291]; Department of Energy [DE-AC05-00OR22725] FX Research conducted at ORNL's Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. The authors acknowledge the Center for Structural Molecular Biology supported by the Office of Biological and Environmental Research (ERKP291). This manuscript has been authored by UT-Battelle, LLC, under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. NR 52 TC 10 Z9 10 U1 2 U2 26 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAR 26 PY 2015 VL 119 IS 12 BP 4460 EP 4470 DI 10.1021/acs.jpcb.5b00220 PG 11 WC Chemistry, Physical SC Chemistry GA CE6TM UT WOS:000351971100012 PM 25738532 ER PT J AU Reichhardt, C Ray, D Reichhardt, CJO AF Reichhardt, C. Ray, D. Reichhardt, C. J. Olson TI Quantized transport for a skyrmion moving on a two-dimensional periodic substrate SO PHYSICAL REVIEW B LA English DT Article ID VORTEX LATTICES; COLLOIDAL MONOLAYERS; MAGNETIC SKYRMIONS; CHIRAL MAGNET; PHASE-LOCKING; MOTION; DRIVEN; STATES; DYNAMICS; SUPERCONDUCTORS AB We examine the dynamics of a skyrmionmoving over a two-dimensional periodic substrate utilizing simulations of a particle-based skyrmion model. We specifically examine the role of the nondissipative Magnus term on the driven motion and the resulting skyrmion velocity-force curves. In the overdamped limit, there is a depinning transition into a sliding state in which the skyrmion moves in the same direction as the external drive. When there is a finite Magnus component in the equation of motion, a skyrmion in the absence of a substrate moves at an angle with respect to the direction of the external driving force. When a periodic substrate is added, the direction of motion or Hall angle of the skyrmion is dependent on the amplitude of the external drive, only approaching the substrate-free limit for higher drives. Due to the underlying symmetry of the substrate the direction of skyrmion motion does not change continuously as a function of drive, but rather forms a series of discrete steps corresponding to integer or rational ratios of the velocity components perpendicular ([V-perpendicular to]) and parallel ([V-||]) to the external drive direction: [V-perpendicular to]/[V-||] = n/m, where n and m are integers. The skyrmion passes through a series of directional locking phases in which the motion is locked to certain symmetry directions of the substrate for fixed intervals of the drive amplitude. Within a given directionally locked phase, the Hall angle remains constant and the skyrmion moves in an orderly fashion through the sample. Signatures of the transitions into and out of these locked phases take the form of pronounced cusps in the skyrmion velocity versus force curves, as well as regions of negative differential mobility in which the net skyrmion velocity decreases with increasing external driving force. The number of steps in the transport curve increases when the relative strength of the Magnus term is increased. We also observe an overshoot phenomena in the directional locking, where the skyrmion motion can lock to a Hall angle greater than the clean limit value and then jump back to the lower value at higher drives. The skyrmion-substrate interactions can also produce a skyrmion acceleration effect in which, due to the nondissipative dynamics, the skyrmion velocity exceeds the value expected to be produced by the external drive. We find that these effects are robust for different types of periodic substrates. Using a simple model for a skyrmion interacting with a single pinning site, we can capture the behavior of the change in the Hall angle with increasing external drive. When the skyrmion moves through the pinning site, its trajectory exhibits a side step phenomenon since the Magnus term induces a curvature in the skyrmion orbit. As the drive increases, this curvature is reduced and the side step effect is also reduced. Increasing the strength of the Magnus term reduces the range of impact parameters over which the skyrmion can be captured by a pinning site, which is one of the reasons that strong Magnus force effects reduce the pinning in skyrmion systems. C1 [Reichhardt, C.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. RP Reichhardt, C (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. OI Reichhardt, Cynthia/0000-0002-3487-5089 FU NNSA of US DOE at LANL [DE-AC52-06NA25396] FX This work was carried out under the auspices of the NNSA of the US DOE at LANL under Contract No. DE-AC52-06NA25396. NR 66 TC 11 Z9 11 U1 1 U2 27 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAR 26 PY 2015 VL 91 IS 10 AR 104426 DI 10.1103/PhysRevB.91.104426 PG 13 WC Physics, Condensed Matter SC Physics GA CE7JY UT WOS:000352016700002 ER PT J AU Zhang, W Jungfleisch, MB Jiang, WJ Liu, YH Pearson, JE te Velthuis, SGE Hoffmann, A Freimuth, F Mokrousov, Y AF Zhang, Wei Jungfleisch, Matthias B. Jiang, Wanjun Liu, Yaohua Pearson, John E. te Velthuis, Suzanne G. E. Hoffmann, Axel Freimuth, Frank Mokrousov, Yuriy TI Reduced spin-Hall effects from magnetic proximity SO PHYSICAL REVIEW B LA English DT Article ID LOCALIZED WANNIER FUNCTIONS; CIRCULAR-DICHROISM; MULTILAYERS; FERROMAGNETISM; TORQUE; PD AB Harnessing spin-orbit coupling for the manipulation of spins and magnetization via electric charge currents is the key objective of spin-orbitronics. Towards this end ferromagnetic materials are combined with nonmagnetic materials with strong spin-orbit coupling (typically involving heavy elements). However, many of the nominally nonmagnetic materials are highly susceptible to magnetic proximity effects, and the role of induced moments for spin transport has been controversial. Here we demonstrate that for Pt and Pd increased induced magnetic moments are correlated with strongly reduced spin-Hall conductivities. This observation finds an intuitive explanation in the development of a spin splitting of the chemical potential and the energy dependence of the intrinsic spin-Hall effect determined by first-principles calculations. This work provides simple guidance towards the optimization of spin current efficiencies for devices based on spin-orbit coupling phenomena. C1 [Zhang, Wei; Jungfleisch, Matthias B.; Jiang, Wanjun; Liu, Yaohua; Pearson, John E.; te Velthuis, Suzanne G. E.; Hoffmann, Axel] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Freimuth, Frank; Mokrousov, Yuriy] Forschungszentrum Julich, Peter Grunberg Inst, D-52425 Julich, Germany. [Freimuth, Frank; Mokrousov, Yuriy] Forschungszentrum Julich, Inst Adv Simulat, D-52425 Julich, Germany. [Freimuth, Frank; Mokrousov, Yuriy] JARA, D-52425 Julich, Germany. RP Zhang, W (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. RI Liu, Yaohua/B-2529-2009; te Velthuis, Suzanne/I-6735-2013; Zhang, Wei/G-1523-2012; Jungfleisch, Matthias Benjamin/G-1069-2015; Jiang, Wanjun/E-6994-2011; Hoffmann, Axel/A-8152-2009 OI Freimuth, Frank/0000-0001-6193-5991; Liu, Yaohua/0000-0002-5867-5065; te Velthuis, Suzanne/0000-0002-1023-8384; Zhang, Wei/0000-0002-5878-3090; Jungfleisch, Matthias Benjamin/0000-0001-8204-3677; Jiang, Wanjun/0000-0003-0918-3862; Hoffmann, Axel/0000-0002-1808-2767 FU US Department of Energy, Office of Science, Materials Science and Engineering Division; DOE, Office of Science, Basic Energy Science [DE-AC02-06CH11357]; HGF-YIG Program of DFG [VH-NG-513, SPP 1538] FX This work was supported by the US Department of Energy, Office of Science, Materials Science and Engineering Division. Lithographic patterning was performed at the Center for Nanoscale Materials, which is supported by DOE, Office of Science, Basic Energy Science under Contract No. DE-AC02-06CH11357. Computing time on the supercomputers JUQUEEN and JUROPA at Julich Supercomputing Center and funding under the HGF-YIG Program VH-NG-513 and SPP 1538 of DFG are gratefully acknowledged. NR 54 TC 19 Z9 19 U1 10 U2 43 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 26 PY 2015 VL 91 IS 11 AR 115316 DI 10.1103/PhysRevB.91.115316 PG 7 WC Physics, Condensed Matter SC Physics GA CE7KI UT WOS:000352017800002 ER PT J AU Turnbull, D Michel, P Ralph, JE Divol, L Ross, JS Hopkins, LFB Kritcher, AL Hinkel, DE Moody, JD AF Turnbull, D. Michel, P. Ralph, J. E. Divol, L. Ross, J. S. Hopkins, L. F. Berzak Kritcher, A. L. Hinkel, D. E. Moody, J. D. TI Multibeam Seeded Brillouin Sidescatter in Inertial Confinement Fusion Experiments SO PHYSICAL REVIEW LETTERS LA English DT Article ID NATIONAL IGNITION FACILITY; PHYSICS BASIS; LASER FUSION; DRIVE; LIGHT; PLASMAS; CAPSULE AB We present the first observations of multibeam weakly seeded Brillouin sidescatter in indirect-drive inertial confinement fusion (ICF) experiments. Two seeding mechanisms have been identified and quantified: specular reflections ("glint") from opposite hemisphere beams, and Brillouin backscatter from neighboring beams with a different angle of incidence. Seeded sidescatter can dominate the overall coupling losses, so understanding this process is crucial for proper accounting of energy deposition and drive symmetry. Glint-seeded scattered light could also be used to probe hydrodynamic conditions inside ICF targets. C1 [Turnbull, D.; Michel, P.; Ralph, J. E.; Divol, L.; Ross, J. S.; Hopkins, L. F. Berzak; Kritcher, A. L.; Hinkel, D. E.; Moody, J. D.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Turnbull, D (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM turnbull2@llnl.gov FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX D. T. would like to thank Nino Landen, Nathan Meezan, and Marilyn Schneider for comments and feedback, as well as Jay Salmonson and Steve MacLaren for allowing ride-along experiments to be conducted within their campaign. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 35 TC 7 Z9 8 U1 2 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 26 PY 2015 VL 114 IS 12 AR 125001 DI 10.1103/PhysRevLett.114.125001 PG 5 WC Physics, Multidisciplinary SC Physics GA CE8EM UT WOS:000352074300007 PM 25860748 ER PT J AU Kokot, G Piet, D Whitesides, GM Aranson, IS Snezhko, A AF Kokot, Gasper Piet, David Whitesides, George M. Aranson, Igor S. Snezhko, Alexey TI Emergence of reconfigurable wires and spinners via dynamic self-assembly SO SCIENTIFIC REPORTS LA English DT Article ID MAGNETIC-LEVITATION; ELECTRIC-FIELDS; NANOSTRUCTURES; NANOPARTICLES; COLLOIDS AB Dissipative colloidal materials use energy to generate and maintain structural complexity. The energy injection rate, and properties of the environment are important control parameters that influence the outcome of dynamic self-assembly. Here we demonstrate that dispersions of magnetic microparticles confined at the air-liquid interface, and energized by a uniaxial in-plane alternating magnetic field, self-assemble into a variety of structures that range from pulsating clusters and single-particle-thick wires to dynamic arrays of spinners (self-assembled short chains) rotating in either direction. The spinners emerge via spontaneous breaking of the uniaxial symmetry of the energizing magnetic field. Demonstration of the formation and disaggregation of particle assemblies suggests strategies to form new meso-scale structures with the potential to perform functions such as mixing and sensing. C1 [Kokot, Gasper] Jozef Stefan Inst, Complex Matter Dept, Ljubljana 1000, Slovenia. [Piet, David; Aranson, Igor S.; Snezhko, Alexey] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Piet, David; Aranson, Igor S.] Northwestern Univ, Dept Engn Sci & Appl Math, Evanston, IL 60208 USA. [Whitesides, George M.] Harvard Univ, Dept Chem & Chem Biol, Cambridge, MA 02138 USA. RP Snezhko, A (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM snezhko@anl.gov FU US DOE, Office of Basic Energy Sciences, Division of Materials Science and Engineering [DE AC02-06CH11357, DE-FG02-00ER45852] FX The research of A.S. and I.S.A. was supported by the US DOE, Office of Basic Energy Sciences, Division of Materials Science and Engineering, under the Contract No. DE AC02-06CH11357. The research of G.M.W. was supported by the US DOE, Office of Basic Energy Sciences, Division of Materials Science and Engineering, under the Contract No. DE-FG02-00ER45852. NR 38 TC 9 Z9 9 U1 10 U2 85 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAR 26 PY 2015 VL 5 AR 9528 DI 10.1038/srep09528 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CE3DV UT WOS:000351706300001 PM 25810144 ER PT J AU Cordova, KE Furukawa, H Yaghi, OM AF Cordova, Kyle E. Furukawa, Hiroyasu Yaghi, Omar M. TI The Development of Global Science SO ACS CENTRAL SCIENCE LA English DT Article ID DEVELOPING-COUNTRIES; DEVELOPING-WORLD; CHEMISTRY; EDUCATION; NATIONS; TIME AB How do we build research capacity throughout the world and capture the great human potential? To us, the answer is rather straightforward: the time-honored tradition of scientific mentoring must be practiced on a wider scale across borders. Herein, we detail the necessity for expanding mentorship to a global scale and provide several important principles to be considered when designing, planning, and implementing programs and centers of research around the world. C1 [Cordova, Kyle E.; Furukawa, Hiroyasu; Yaghi, Omar M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Chem, Mat Sci Div,Kavli Energy NanoSci Inst, Berkeley, CA 94720 USA. [Cordova, Kyle E.; Furukawa, Hiroyasu; Yaghi, Omar M.] Ctr Global Sci, Berkeley, CA 94720 USA. [Cordova, Kyle E.; Furukawa, Hiroyasu; Yaghi, Omar M.] Vietnam Natl Univ, Ctr Mol & NanoArchitecture, Ho Chi Minh City 721337, Vietnam. [Furukawa, Hiroyasu; Yaghi, Omar M.] King Fahd Univ Petr & Minerals, Dhahran 34464, Saudi Arabia. [Furukawa, Hiroyasu; Yaghi, Omar M.] Univ Calif Berkeley, Ctr Nanomat Clean Energy Applicat, King Abdulaziz City Sci & Technol, Riyadh 11442, Saudi Arabia. [Yaghi, Omar M.] Natl Inst Mat Sci, Int Ctr Mat Nanoarchitecton WPI MANA, Tsukuba, Ibaraki 3050044, Japan. [Yaghi, Omar M.] Korea Adv Inst Sci & Technol, Grad Sch Energy Environm Water & Sustainabil, Taejon 305701, South Korea. RP Yaghi, OM (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Chem, Mat Sci Div,Kavli Energy NanoSci Inst, Berkeley, CA 94720 USA. EM yaghi@berkeley.edu RI Furukawa, Hiroyasu/C-5910-2008; OI Furukawa, Hiroyasu/0000-0002-6082-1738; Cordova, Kyle/0000-0002-4988-0497 NR 24 TC 2 Z9 2 U1 4 U2 14 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2374-7943 EI 2374-7951 J9 ACS CENTRAL SCI JI ACS Central Sci. PD MAR 25 PY 2015 VL 1 IS 1 BP 18 EP 23 DI 10.1021/acscentsci.5b00028 PG 6 WC Chemistry, Multidisciplinary SC Chemistry GA CV3LA UT WOS:000364159500008 PM 27162942 ER PT J AU Chen, Q Cho, H Manthiram, K Yoshida, M Ye, XC Alivisatos, AP AF Chen, Qian Cho, Hoduk Manthiram, Karthish Yoshida, Mark Ye, Xingchen Alivisatos, A. Paul TI Interaction Potentials of Anisotropic Nanocrystals from the Trajectory Sampling of Particle Motion using in Situ Liquid Phase Transmission Electron Microscopy SO ACS CENTRAL SCIENCE LA English DT Article ID GOLD NANORODS; SILVER NANOPARTICLES; GROWTH; CLUSTERS; FORCES; AGGREGATION; LATTICES; CELLS AB We demonstrate a generalizable strategy to use the relative trajectories of pairs and groups of nanocrystals, and potentially other nanoscale objects, moving in solution which can now be obtained by in situ liquid phase transmission electron microscopy (TEM) to determine the interaction potentials between nanocrystals. Such nanoscale interactions are crucial for collective behaviors and applications of synthetic nanocrystals and natural biomolecules, but have been very challenging to measure in situ at nanometer or sub-nanometer resolution. Here we use liquid phase TEM to extract the mathematical form of interaction potential between nanocrystals from their sampled trajectories. We show the power of this approach to reveal unanticipated features of nanocrystal-nanocrystal interactions by examining the anisotropic interaction potential between charged rod-shaped Au nanocrystals (Au nanorods); these Au nanorods assemble, in a tip-to-tip fashion in the liquid phase, in contrast to the well-known side-by-side arrangements commonly observed for drying-mediated assembly. These observations can be explained by a long-range and highly anisotropic electrostatic repulsion that leads to the tip-selective attachment. As a result, Au nanorods stay unassembled at a lower ionic strength, as the electrostatic repulsion is even longer-ranged. Our study not only provides a mechanistic understanding of the process by which metallic nanocrystals assemble but also demonstrates a method that can potentially quantify and elucidate a broad range of nanoscale interactions relevant to nanotechnology and biophysics. C1 [Chen, Qian] Univ Calif Berkeley, Miller Inst Basic Res Sci, Berkeley, CA 94720 USA. [Chen, Qian; Cho, Hoduk; Ye, Xingchen; Alivisatos, A. Paul] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Alivisatos, A. Paul] Univ Calif Berkeley, Kavli Energy NanoSci Inst, Berkeley, CA 94720 USA. [Manthiram, Karthish; Yoshida, Mark] Univ Calif Berkeley, Dept Chem Engn, Berkeley, CA 94720 USA. [Chen, Qian; Cho, Hoduk; Manthiram, Karthish; Ye, Xingchen; Alivisatos, A. Paul] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Cho, Hoduk; Alivisatos, A. Paul] King Abdulaziz City Sci & Technol, Riyadh, Saudi Arabia. RP Alivisatos, AP (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM alivis@berkeley.edu RI Alivisatos , Paul /N-8863-2015; Ye, Xingchen/D-3202-2017; OI Alivisatos , Paul /0000-0001-6895-9048; Ye, Xingchen/0000-0001-6851-2721; Cho, Hoduk/0000-0002-0082-0637 NR 53 TC 32 Z9 32 U1 19 U2 37 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2374-7943 EI 2374-7951 J9 ACS CENTRAL SCI JI ACS Central Sci. PD MAR 25 PY 2015 VL 1 IS 1 BP 33 EP 39 DI 10.1021/acscentsci.5b00001 PG 7 WC Chemistry, Multidisciplinary SC Chemistry GA CV3LA UT WOS:000364159500010 PM 27162944 ER PT J AU Ewbank, JL Kovarik, L Diallo, FZ Sievers, C AF Ewbank, Jessica L. Kovarik, Libor Diallo, Fatoumata Z. Sievers, Carsten TI Effect of metal-support interactions in Ni/Al2O3 catalysts with low metal loading for methane dry reforming SO APPLIED CATALYSIS A-GENERAL LA English DT Article DE Rational synthesis; Nickel; Alumina; Adsorption; Metal-support interactions ID NICKEL-ALUMINA CATALYSTS; TEMPERATURE-PROGRAMMED-REDUCTION; HIGHLY DISPERSED NOBLE; CHEMICAL-STRUCTURES; CARBON-DIOXIDE; GAMMA-ALUMINA; ELECTRON-MICROSCOPY; THERMAL-STABILITY; SURFACE-AREA; NI CATALYSTS AB Nickel catalysts prepared by a variety of different methods are commonly used for reforming reactions such as methane dry reforming. Two preparation methods, controlled adsorption and dry impregnation, are implemented to explore the effect of preparation method on the formation of active sites on alumina supported nickel catalysts. By varying only the preparation method, comparison of catalysts that differ primarily in metal-support interactions, strong metal-support interaction (controlled adsorption) and weak metal-support interactions (dry impregnation), are obtained. For controlled adsorption, optimal synthesis conditions are identified using point of zero charge measurements, pH-precipitation experiments, and adsorption isotherms. Using these conditions, a catalyst with a higher dispersion and strong metal-support interactions is prepared. Physicochemical characterization by N-2 physisorption, H-2 chemisorption, temperature programmed reduction (TPR), transmission electron microscopy (TEM), and environmental TEM (ETEM) shows that the types of nickel sites formed strongly depend on the synthesis method. Methane dry reforming reactivity studies show stable catalytic performance for at least 9 h and provide additional insight into the types of active centers present. After reductive pretreatment, the nickel catalyst prepared by dry impregnation is found to primarily have nickel present as a surface NiAl2O4. In contrast, the active centers for the nickel catalyst prepared by controlled adsorption consist of nickel particles that are encapsulated by a nickel aluminate layer with 1-2 nm in thickness. Combustion analysis and XPS of spent catalysts reveal different amounts and nature of carbonaceous deposits as a function of the synthesis method. (C) 2015 Elsevier B.V. All rights reserved. C1 [Ewbank, Jessica L.; Diallo, Fatoumata Z.; Sievers, Carsten] Georgia Inst Technol, Sch Chem & Biomol Engn, Atlanta, GA 30332 USA. [Ewbank, Jessica L.; Sievers, Carsten] Georgia Inst Technol, Renewable Bioprod Inst, Atlanta, GA 30332 USA. [Kovarik, Libor] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. RP Sievers, C (reprint author), Georgia Inst Technol, Sch Chem & Biomol Engn, Atlanta, GA 30332 USA. EM carsten.sievers@chbe.gatech.edu RI Kovarik, Libor/L-7139-2016 FU Dow Chemical Company; Renewable Bioproducts Institute at the Georgia Institute of Technology; DOE's Office of Biological and Environmental Research FX The authors wish to thank Micromeritics Corporation and Jeff Kenvin for TPR and H2 chemisorption measurements. Funding from The Dow Chemical Company and the Renewable Bioproducts Institute at the Georgia Institute of Technology is gratefully acknowledged. Transmission Electron Microscopy measurements described in this paper were conducted in the William R. Wiley Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by DOE's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. We thank John R. Regalbuto for guidance on Strong Electrostatic Adsorption (SEA). NR 59 TC 19 Z9 19 U1 20 U2 110 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0926-860X EI 1873-3875 J9 APPL CATAL A-GEN JI Appl. Catal. A-Gen. PD MAR 25 PY 2015 VL 494 BP 57 EP 67 DI 10.1016/j.apcata.2015.01.029 PG 11 WC Chemistry, Physical; Environmental Sciences SC Chemistry; Environmental Sciences & Ecology GA CF9ZN UT WOS:000352926500007 ER PT J AU Li, Q Pan, HY Higgins, D Cao, RG Zhang, GQ Lv, HF Wu, KB Cho, J Wu, G AF Li, Qing Pan, Hengyu Higgins, Drew Cao, Ruiguo Zhang, Guoqi Lv, Haifeng Wu, Kangbing Cho, Jaephil Wu, Gang TI Metal-Organic Framework-Derived Bamboo-like Nitrogen-Doped Graphene Tubes as an Active Matrix for Hybrid Oxygen-Reduction Electrocatalysts SO SMALL LA English DT Article ID ELECTROLYTE FUEL-CELLS; CARBON-NANOTUBE; METHANOL OXIDATION; EFFICIENT ELECTROCATALYSTS; LI-O-2 BATTERIES; CATALYSTS; IRON; PLATINUM; NANOCOMPOSITES; NANOPARTICLES AB In this work, large size (i.e., diameter > 100 nm) graphene tubes with nitrogen-doping are prepared through a high-temperature graphitization process of dicyandiamide (DCDA) and Iron(II) acetate templated by a novel metal-organic framework (MIL-100(Fe)). The nitrogen-doped graphene tube (N-GT)-rich iron-nitrogen-carbon (Fe-N-C) catalysts exhibit inherently high activity towards the oxygen reduction reaction (ORR) in more challenging acidic media. Furthermore, aiming to improve the activity and stability of conventional Pt catalysts, the ORR active N-GT is used as a matrix to disperse Pt nanoparticles in order to build a unique hybrid Pt cathode catalyst. This is the first demonstration of the integration of a highly active Fe-N-C catalyst with Pt nanoparticles. The synthesized 20% Pt/N-GT composite catalysts demonstrate significantly enhanced ORR activity and H-2-air fuel cell performance relative to those of 20% Pt/C, which is mainly attributed to the intrinsically active N-GT matrix along with possible synergistic effects between the non-precious metal active sites and the Pt nanoparticles. Unlike traditional Pt/C, the hybrid catalysts exhibit excellent stability during the accelerated durability testing, likely due to the unique highly graphitized graphene tube morphologies, capable of providing strong interaction with Pt nanoparticles and then preventing their agglomeration. C1 [Li, Qing; Higgins, Drew] Los Alamos Natl Lab, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA. [Pan, Hengyu; Wu, Gang] SUNY Buffalo, Dept Chem & Biol Engn, Buffalo, NY 14260 USA. [Cao, Ruiguo; Cho, Jaephil] Ulsan Natl Inst Sci & Technol, Interdisciplinary Sch Green Energy, Ulsan 689798, South Korea. [Zhang, Guoqi] CUNY John Jay Coll Criminal Justice, Dept Sci, New York, NY 10019 USA. [Lv, Haifeng] Wuhan Univ Technol, State Key Lab Adv Technol Mat Synth & Proc, Wuhan 430070, Peoples R China. [Wu, Kangbing] Huazhong Univ Sci & Technol, Key Lab Large Format Battery Mat & Syst, Minist Educ, Sch Chem & Chem Engn, Wuhan 430074, Peoples R China. RP Cho, J (reprint author), Ulsan Natl Inst Sci & Technol, Interdisciplinary Sch Green Energy, Ulsan 689798, South Korea. EM jpcho@unist.ac.kr; gangwu@buffalo.edu RI Cho, Jaephil/E-4265-2010; Li, Qing/G-4502-2011; Wu, Gang/E-8536-2010; Cao, Ruiguo/O-7354-2016 OI Li, Qing/0000-0003-4807-030X; Wu, Gang/0000-0003-4956-5208; FU University at Buffalo, SUNY; LDRD Program of Los Alamos National Laboratory; National Basic Research Program of China (973 Program) [2015CB352100]; MSIP (Ministry of Science, ICT & Future Planning), Korea, under the C-ITRC (Convergence Information Technology Research Center) [NIPA-2013-H0301-13-1009] FX G. W. acknowledges the financial support from the start-up funding of University at Buffalo, SUNY along with the LDRD Program of Los Alamos National Laboratory. H. L. thanks the National Basic Research Program of China (973 Program, No. 2015CB352100) for supporting this work. J.P C also thanks the financial supports by the MSIP (Ministry of Science, ICT & Future Planning), Korea, under the C-ITRC (Convergence Information Technology Research Center) support program (NIPA-2013-H0301-13-1009) supervised by the NIPA (National IT Industry Promotion Agency). NR 52 TC 43 Z9 43 U1 43 U2 284 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1613-6810 EI 1613-6829 J9 SMALL JI Small PD MAR 25 PY 2015 VL 11 IS 12 BP 1443 EP 1452 DI 10.1002/smll.201402069 PG 10 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CF4WK UT WOS:000352553600012 PM 25400088 ER PT J AU Acharya, KP Nguyen, HM Paulite, M Piryatinski, A Zhang, J Casson, JL Xu, HW Htoon, H Hollingsworth, JA AF Acharya, Krishna P. Nguyen, Hue M. Paulite, Melissa Piryatinski, Andrei Zhang, Jun Casson, Joanna L. Xu, Hongwu Htoon, Han Hollingsworth, Jennifer A. TI Elucidation of Two Giants: Challenges to Thick-Shell Synthesis in CdSe/ZnSe and ZnSe/CdS Core/Shell Quantum Dots SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID SEMICONDUCTOR NANOCRYSTALS; SUPPRESSED BLINKING; LUMINESCENCE; EMISSION; GAIN AB Core/thick-shell giant quantum dots (gQDs) possessing type II electronic structures exhibit suppressed blinking and diminished nonradiative Anger recombination. We investigate CdSe/ZnSe and ZASe/CdS as potential new gQDs. We Show theoretically and experimentally that both can exhibit partial or complete spatial separation of an excited-state electron hole pair (i.e., type II behavior). However; we reveal that thick-shell growth is challenged by competing processes: alloying and cation exchange. We demonstrate that these can be largely avoided by choice of shelling conditions (e.g., time, temperature, and QD core identity). The resulting CdSe/ZnSe gQDs exhibit unusual single-QD properties, principally emitting from dim gray states but having high two-exciton (biexciton) emission efficiencies, whereas ZnSe/CdS gQDs show characteristic gQD blinking suppression, though only if shelling is accompanied by partial cation exchange. C1 [Acharya, Krishna P.; Nguyen, Hue M.; Paulite, Melissa; Htoon, Han; Hollingsworth, Jennifer A.] Los Alamos Natl Lab, Mat Phys & Applicat Div, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. [Piryatinski, Andrei] Los Alamos Natl Lab, Div Theoret, Phys Condensed Matter & Complex Syst, Los Alamos, NM 87545 USA. [Zhang, Jun; Xu, Hongwu] Los Alamos Natl Lab, Earth & Environm Sci Div, Earth Syst Observat, Los Alamos, NM 87545 USA. [Casson, Joanna L.] Los Alamos Natl Lab, Chem Div, Phys Chem & Appl Spect, Los Alamos, NM 87545 USA. RP Hollingsworth, JA (reprint author), Los Alamos Natl Lab, Mat Phys & Applicat Div, Ctr Integrated Nanotechnol, POB 1663, Los Alamos, NM 87545 USA. EM jenn@lanl.gov RI Piryatinski, Andrei/B-5543-2009; OI Xu, Hongwu/0000-0002-0793-6923; Htoon, Han/0000-0003-3696-2896 FU Division of Materials Science and Engineering, Office of Basic Energy Sciences (OBES), Office of Science, U.S. Department of Energy (DOE) [2009LANL1096] FX Funding from a Division of Materials Science and Engineering, Office of Basic Energy Sciences (OBES), Office of Science, U.S. Department of Energy (DOE) grant (2009LANL1096). Work performed largely at CINT, a DOE/OBES Nanoscale Science Research Center & User Facility. We thank D. Williams for obtaining XRDs. NR 30 TC 12 Z9 12 U1 14 U2 136 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAR 25 PY 2015 VL 137 IS 11 BP 3755 EP 3758 DI 10.1021/jacs.5b00313 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA CE6TV UT WOS:000351972000008 PM 25746140 ER PT J AU Fox, JM Kang, K Sherman, W Heroux, A Sastry, GM Baghbanzadeh, M Lockett, MR Whitesides, GM AF Fox, Jerome M. Kang, Kyungtae Sherman, Woody Heroux, Annie Sastry, G. Madhavi Baghbanzadeh, Mostafa Lockett, Matthew R. Whitesides, George M. TI Interactions between Hofmeister Anions and the Binding Pocket of a Protein SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID CARBONIC-ANHYDRASE-II; INHOMOGENEOUS FLUID APPROACH; LIGAND-BINDING; SOLVATION THERMODYNAMICS; BIOLOGICAL STRUCTURE; SURFACE-TENSION; SALT-SOLUTIONS; ION CHANNELS; WATER; MACROMOLECULES AB This paper uses the binding pocket of human carbonic anhydrase II (HCAII, EC 4.2.1.1) as a tool to examine the properties of Hofmeister anions that determine (i) where, and how strongly, they associate with concavities on the surfaces of proteins and (ii) how, upon binding, they alter the structure of water within those concavities. Results from X-ray crystallography and isothermal titration calorimetry show that most anions associate with the binding pocket of HCAII by forming inner-sphere ion pairs with the Zn2+ cofactor. In these ion pairs, the free energy of anion-Zn2+ association is inversely proportional to the free energetic cost of anion dehydration; this relationship is consistent with the mechanism of ion pair formation suggested by the "law of matching water affinities". Iodide and bromide anions also associate with a hydrophobic declivity in the wall of the binding pocket. Molecular dynamics simulations suggest that anions, upon associating with Zn2+, trigger rearrangements of water that extend up to 8 A away from their surfaces. These findings expand the range of interactions previously thought to occur between ions and proteins by suggesting that (i) weakly hydrated anions can bind complementarily shaped hydrophobic declivities, and that (ii) ion-induced rearrangements of water within protein concavities can (in contrast with similar rearrangements in bulk water) extend well beyond the first hydration shells of the ions that trigger them. This study paints a picture of Hofmeister anions as a set of structurally varied ligands that differ in size, shape, and affinity for water and, thus, in their ability to bind to and to alter the charge and hydration structure of polar, nonpolar, and topographically complex concavities on the surfaces of proteins. C1 [Fox, Jerome M.; Kang, Kyungtae; Baghbanzadeh, Mostafa; Lockett, Matthew R.; Whitesides, George M.] Harvard Univ, Dept Chem & Chem Biol, Cambridge, MA 02138 USA. [Whitesides, George M.] Harvard Univ, Wyss Inst Biol Inspired Engn, Cambridge, MA 02138 USA. [Whitesides, George M.] Harvard Univ, Kavli Inst Bionano Sci & Technol, Cambridge, MA 02138 USA. [Sherman, Woody] Schrodinger, New York, NY 10036 USA. [Heroux, Annie] Brookhaven Natl Lab, Photon Sci Div, Energy Sci Directorate, Upton, NY 11937 USA. [Sastry, G. Madhavi] Schrodinger, Hyderabad 11937, Andhra Pradesh, India. RP Whitesides, GM (reprint author), Harvard Univ, Dept Chem & Chem Biol, 12 Oxford St, Cambridge, MA 02138 USA. EM gwhitesides@gmwgroup.harvard.edu RI Lockett, Matthew/A-6020-2015; OI Lockett, Matthew/0000-0003-4851-7757; FOX, JEROME/0000-0002-3739-1899 FU National Science Foundation [1152196]; NIH/NIGMS [8P41GM103473-16]; DOE/BER [BO-70]; DOE/BES [DE-AC02-98CH10886] FX We thank Serena Bai and Phil Snyder (Harvard University) for initial X-ray crystallography studies of the association of iodide and the binding pocket of HCAII, and Benjamin Breiten (Harvard University) for helpful discussions. This work was supported by the National Science Foundation under Award No. 1152196. A.H. was additionally supported by NIH/NIGMS grant 8P41GM103473-16 and DOE/BER grant BO-70. Structural data were collected at beamline X25 of the National Synchrotron Light Source under support of DOE/BES Contract No. DE-AC02-98CH10886. NR 78 TC 20 Z9 20 U1 6 U2 81 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAR 25 PY 2015 VL 137 IS 11 BP 3859 EP 3866 DI 10.1021/jacs.5b00187 PG 8 WC Chemistry, Multidisciplinary SC Chemistry GA CE6TV UT WOS:000351972000027 PM 25738615 ER PT J AU Shanavas, KV Singh, DJ AF Shanavas, K. V. Singh, David J. TI Itinerant Magnetism in Metallic CuFe2Ge2 SO PLOS ONE LA English DT Article AB Theoretical calculations are performed to understand the electronic structure and magnetic properties of CuFe2Ge2. The band structure reveals large electron density N(E-F) at the Fermi level suggesting a strong itinerant character of magnetism. The Fermi surface is dominated by two dimensional sheet like structures, with potentially strong nesting between them. The magnetic ground state appears to be ferromagnetic along a and antiferromagnetic in other directions. These results show that CuFe2Ge2 is an antiferromagnetic metal, with similarities to the Fe-based superconductors; such as magnetism with substantial itinerant character and coupling between magnetic order and electrons at the Fermi energy. C1 [Shanavas, K. V.; Singh, David J.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Shanavas, KV (reprint author), Oak Ridge Natl Lab, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. EM kavungalvees@ornl.gov FU United States Department of Energy, Basic Energy Sciences, Office of Science, Materials Sciences and Engineering Division FX This research was supported by the United States Department of Energy, Basic Energy Sciences, Office of Science, Materials Sciences and Engineering Division. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 17 TC 2 Z9 2 U1 3 U2 14 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAR 25 PY 2015 VL 10 IS 3 AR e0121186 DI 10.1371/journal.pone.0121186 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CE5MO UT WOS:000351880000134 PM 25807140 ER PT J AU Techtmann, SM Fortney, JL Ayers, KA Joyner, DC Linley, TD Pfiffner, SM Hazen, TC AF Techtmann, Stephen M. Fortney, Julian L. Ayers, Kati A. Joyner, Dominique C. Linley, Thomas D. Pfiffner, Susan M. Hazen, Terry C. TI The Unique Chemistry of Eastern Mediterranean Water Masses Selects for Distinct Microbial Communities by Depth SO PLOS ONE LA English DT Article ID DEEP-SEA FAN; PHOSPHORUS STARVATION; BACTERIAL COMMUNITIES; NATURAL WATERS; ASSEMBLAGES; LIMITATION; OCEAN; PROCHLOROCOCCUS; OXIDATION; SEDIMENT AB The waters of the Eastern Mediterranean are characterized by unique physical and chemical properties within separate water masses occupying different depths. Distinct water masses are present throughout the oceans, which drive thermohaline circulation. These water masses may contain specific microbial assemblages. The goal of this study was to examine the effect of physical and geological phenomena on the microbial community of the Eastern Mediterranean water column. Chemical measurements were combined with phospholipid fatty acid (PLFA) analysis and high-throughput 16S rRNA sequencing to characterize the microbial community in the water column at five sites. We demonstrate that the chemistry and microbial community of the water column were stratified into three distinct water masses. The salinity and nutrient concentrations vary between these water masses. Nutrient concentrations increased with depth, and salinity was highest in the intermediate water mass. Our PLFA analysis indicated different lipid classes were abundant in each water mass, suggesting that distinct groups of microbes inhabit these water masses. 16S rRNA gene sequencing confirmed the presence of distinct microbial communities in each water mass. Taxa involved in autotrophic nitrogen cycling were enriched in the intermediate water mass suggesting that microbes in this water mass may be important to the nitrogen cycle of the Eastern Mediterranean. The Eastern Mediterranean also contains numerous active hydrocarbon seeps. We sampled above the North Alex Mud Volcano, in order to test the effect of these geological features on the microbial community in the adjacent water column. The community in the waters overlaying the mud volcano was distinct from other communities collected at similar depths and was enriched in known hydrocarbon degrading taxa. Our results demonstrate that physical phenomena such stratification as well as geological phenomena such as mud volcanoes strongly affect microbial community structure in the Eastern Mediterranean water column. C1 [Techtmann, Stephen M.; Fortney, Julian L.; Joyner, Dominique C.; Hazen, Terry C.] Univ Tennessee, Dept Civil & Environm Engn, Knoxville, TN 37996 USA. [Techtmann, Stephen M.; Fortney, Julian L.; Ayers, Kati A.; Joyner, Dominique C.; Pfiffner, Susan M.; Hazen, Terry C.] Univ Tennessee, Ctr Environm Biotechnol, Knoxville, TN 37932 USA. [Ayers, Kati A.; Hazen, Terry C.] Univ Tennessee, Dept Earth & Planetary Sci, Knoxville, TN USA. [Linley, Thomas D.] Univ Aberdeen, Ocean Lab, Newburgh, Aberdeen, Scotland. [Pfiffner, Susan M.; Hazen, Terry C.] Univ Tennessee, Dept Microbiol, Knoxville, TN 37996 USA. [Hazen, Terry C.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN USA. RP Techtmann, SM (reprint author), Univ Tennessee, Dept Civil & Environm Engn, Knoxville, TN 37996 USA. EM stephen.techtmann@gmail.com RI Hazen, Terry/C-1076-2012 OI Hazen, Terry/0000-0002-2536-9993 FU University of Tennessee [A13-0119-001]; BP America [A13-0119-001] FX This research was supported by contract A13-0119-001 Deep Sea Basin Microbiology between the University of Tennessee and BP America. The sponsors helped to organize sample collection but had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 81 TC 4 Z9 5 U1 1 U2 22 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAR 25 PY 2015 VL 10 IS 3 AR e0120605 DI 10.1371/journal.pone.0120605 PG 22 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CE5MO UT WOS:000351880000090 PM 25807542 ER PT J AU Reynolds, JG Carter, R Felmy, AR AF Reynolds, Jacob G. Carter, Robert Felmy, Andrew R. TI A Pitzer Interaction Model for the NaNO3-NaNO2-NaOH-H2O System from 0 to 100 degrees C SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID AQUEOUS THERMODYNAMIC MODEL; HIGH-IONIC-STRENGTH; SODIUM-NITRATE; CALCIUM-CHLORIDE; VAPOR-PRESSURES; NATURAL-WATERS; ISOPIESTIC DETERMINATION; ACTIVITY-COEFFICIENTS; OSMOTIC COEFFICIENTS; SOLUBILITY PRODUCT AB The solubility relations and water activities in NaNO3, NaNO2, and NaOH solutions are used in many applications, including the management of alkaline high-level nuclear waste. Only limited water activity data is available at temperatures above ambient for NaNO3 and NaNO2 aqueous solutions, so water activity was-Measured 'by isopiestic methods at 50 and 100 degrees C in this study. The results are consistent with the limited experimentil data previously available. These data are used to parameterize the Pitzer electrolyte solution model for these electrolytes and NaOH in water between 0 and 100 degrees C. Neutral ion pairs between Na+ and NO3+ as well as Na+ and NO2 were required in Order to fit the data adequately. Ternary Pitzer ion interaction parameters for the interactions between the electrolytes were also required and developed to model s,olubility in mixtures of the electrolytes: These results provide,a strong foundation for modelirig the effect of NaNO2, NaNO3, and NaOH on the solubility of other key electrolytes of interest to the management of high-level nuclear waste. C1 [Reynolds, Jacob G.] Washington River Protect Solut LLC, Richland, WA 99352 USA. [Carter, Robert] EnergySolutions, Salt Lake City, UT 84101 USA. [Felmy, Andrew R.] Pacific NW Natl Lab, Richland, WA 99354 USA. RP Reynolds, JG (reprint author), Washington River Protect Solut LLC, POB 850 MSIN H6-04, Richland, WA 99352 USA. EM jacob_g_reynolds@rl.gov NR 69 TC 6 Z9 7 U1 3 U2 10 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD MAR 25 PY 2015 VL 54 IS 11 BP 3062 EP 3070 DI 10.1021/acs.iecr.5b00016 PG 9 WC Engineering, Chemical SC Engineering GA CE6UB UT WOS:000351972600025 ER PT J AU Lentz, M Klaus, M Wagner, M Fahrenson, C Beyerlein, IJ Zecevic, M Reimers, W Knezevic, M AF Lentz, Martin Klaus, Manuela Wagner, Michael Fahrenson, Christoph Beyerlein, Irene J. Zecevic, Milovan Reimers, Walter Knezevic, Marko TI Effect of age hardening on the deformation behavior of an Mg-Y-Nd alloy: In-situ X-ray diffraction and crystal plasticity modeling SO MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING LA English DT Article DE Magnesium alloys; Crystal plasticity; In-situ diffraction; Deformation behavior; Texture ID MAGNESIUM ALLOY; TEXTURE EVOLUTION; GRAIN-SIZE; RARE-EARTH; POLYCRYSTAL PLASTICITY; MECHANICAL RESPONSE; NEUTRON-DIFFRACTION; PRECIPITATE SHAPE; TWIN NUCLEATION; ALPHA-URANIUM AB The present study investigates the deformation behavior of an extruded Mg-Y-Nd (WE54) alloy in as-extruded and aged conditions. Via age-hardening at 250 degrees C for 16 and 500 h or annealing treatments at 400 degrees C for 24 h, precipitates are formed within the grains or at the grain boundaries. To characterize microstructural changes with the age-hardening conditions, we employ electron-backscattered diffraction, transmission electron microscopy, and optical microscopy. In the as-extruded material, we observed an uncommonly low activity of {10 (1) over bar2}< 10 (11) over bar > tension twinning in comparison with other Mg alloys. The tension twinning activity substantially increased after precipitation hardening and the accompanying reduction of alloying element concentration in solid solution. Consistent with the microstructural observations, the increase in twin activity clearly manifests in the compression flow curves. While the as-extruded and 16 h/250 degrees C samples exhibited a classical decreasing hardening rate throughout straining associated with crystallographic slip, the 500 h/250 degrees C and the 400 degrees C annealed sample featured a characteristic increase in the hardening rate associated with twinning. In order to determine the impact of the different heat treatments on the individual slip and twinning modes, in-situ energy-dispersive X-ray synchrotron diffraction experiments during loading and elasto-plastic self-consistent modeling were conducted. We find that plate-shape precipitates on the {10 (1) over bar0}(alpha), planes harden < a > basal slip more than the other slip systems, while the reduced solute concentration in the 500 h 250 degrees C and 24 h 400 degrees C samples results in a significant decrease in the critical resolved shear stress for {10 (1) over bar2}< 10 (11) over bar > tension twinning. (C) 2015 Elsevier B.V. All rights reserved. C1 [Lentz, Martin; Wagner, Michael; Reimers, Walter] Tech Univ Berlin, Metall Werkstoffe, D-10587 Berlin, Germany. [Klaus, Manuela] Helmholtz Zentrum Berlin Mat & Energien, D-12489 Berlin, Germany. [Fahrenson, Christoph] Tech Univ Berlin, Zentraleinrichtung Elektronenmikroskopie, D-10623 Berlin, Germany. [Beyerlein, Irene J.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Zecevic, Milovan; Knezevic, Marko] Univ New Hampshire, Dept Mech Engn, Durham, NH 03824 USA. RP Lentz, M (reprint author), Tech Univ Berlin, Metall Werkstoffe, Ernst Reuter Pl 1, D-10587 Berlin, Germany. EM martin.lentz@tu-berlin.de RI Beyerlein, Irene/A-4676-2011; OI Lentz, Martin/0000-0001-8310-0063 FU Deutsche Forschungsgemeinschaft (DFG) [RE 688/67-1]; U.S. National Science Foundation [CMMI-1301081]; Laboratory Directed Research and Development [20140348ER] FX M. Lentz and W. Reimers are grateful for the financial support of the Deutsche Forschungsgemeinschaft (DFG) under the Contract no. RE 688/67-1. M. Knezevic and M. Zecevic were supported by a U.S. National Science Foundation Grant CMMI-1301081. I.J. Beyerlein gratefully acknowledges support by a Laboratory Directed Research and Development project 20140348ER. The authors would like to thank Katrin Brommelhoff, Alexander Treff and Christoph Seyfert (TU Berlin, Metallische Werkstoffe) for the support of the in-situ experiments, Soren Selve (TU Berlin, ZELMI) for conducting the HR-TEM analysis and Jorg Nissen (TU Berlin, ZELMI) for conducting the EPMA analysis. NR 73 TC 21 Z9 21 U1 3 U2 34 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0921-5093 EI 1873-4936 J9 MAT SCI ENG A-STRUCT JI Mater. Sci. Eng. A-Struct. Mater. Prop. Microstruct. Process. PD MAR 25 PY 2015 VL 628 BP 396 EP 409 DI 10.1016/j.msea.2015.01.069 PG 14 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA CE6RN UT WOS:000351965800049 ER PT J AU Beiersdorfer, P Brown, GV AF Beiersdorfer, Peter Brown, Gregory V. TI Experimental study of the x-ray transitions in the heliumlike isoelectronic sequence: Updated results SO PHYSICAL REVIEW A LA English DT Article ID BEAM ION-TRAP; HIGHLY-CHARGED IONS; CONFIGURATION-INTERACTION CALCULATIONS; HE-LIKE IONS; ELECTRON-BEAM; WAVELENGTH MEASUREMENTS; CROSS-SECTIONS; ENERGY-LEVEL; LAMB SHIFT; FE-XXV AB We revisit the discrepancy between experiments and theory for the x-ray transitions of heliumlike ions and report on a measurement of the n = 2 -> n = 1 x-ray transitions of heliumlike Cu27+. These measurements were carried at the Livermore electron beam ion trap facility and achieved an accuracy of 18 ppm. The measured values show reasonable agreement with theory, but they do not follow the trend established by other measurements with similar uncertainties. C1 [Beiersdorfer, Peter; Brown, Gregory V.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Beiersdorfer, P (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; LLNL LDRD [12-LW-026] FX This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344 and supported in part by LLNL LDRD Project No. 12-LW-026. NR 59 TC 3 Z9 3 U1 1 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9926 EI 2469-9934 J9 PHYS REV A JI Phys. Rev. A PD MAR 25 PY 2015 VL 91 IS 3 AR 032514 DI 10.1103/PhysRevA.91.032514 PG 6 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA CE5KW UT WOS:000351874400008 ER PT J AU Kas, JJ Vila, FD Rehr, JJ Chambers, SA AF Kas, J. J. Vila, F. D. Rehr, J. J. Chambers, S. A. TI Real-time cumulant approach for charge-transfer satellites in x-ray photoemission spectra SO PHYSICAL REVIEW B LA English DT Article ID CORE-LEVEL PHOTOEMISSION; PLASMON SATELLITES; SUDDEN LIMIT; NIO; APPROXIMATION; PHOTOELECTRON; SINGULARITIES; EXCITATIONS; TRANSITION; METALS AB X-ray photoemission spectra generally exhibit satellite features beyond the main peak due to many-body excitations. However, the satellites associated with charge-transfer excitations in correlatedmaterials have proved difficult to calculate from first principles and their interpretation has been controversial. Here we show that these satellites can be attributed to local density fluctuations in response to a suddenly created core hole. Our approach is based on a cumulant representation of the core-hole Green's function with a real-time, time-dependent density functional theory calculation of the cumulant. This approach includes effects that cannot be accounted for by cluster methods and yields a direct real-space, real-time interpretation. Illustrative results for TiO2 and NiO are in good agreement with XPS experiment. C1 [Kas, J. J.; Vila, F. D.; Rehr, J. J.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Chambers, S. A.] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. RP Kas, JJ (reprint author), Univ Washington, Dept Phys, Seattle, WA 98195 USA. FU DOE [DE-FG03-97ER45623]; DOE BES DMSE [10122] FX We thank P. Bagus, G. Bertsch, J. Freericks, A. Lee, and L. Reining for useful comments. This work was supported by DOE Grant No. DE-FG03-97ER45623 (J.J.R. and J.J.K.) and DOE BES DMSE Award No. 10122 (S.A.C.), and was facilitated by the DOE Computational Materials Science Network. One of us (J.J.R.) also thanks the the Kavli Institute for Theoretical Physics at UCSB and the Laboratoire des Solides Irradies, Ecole Polytechnique, CNRS, Palaiseau, France for hospitality where parts of this work were carried out. NR 45 TC 8 Z9 8 U1 3 U2 18 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAR 25 PY 2015 VL 91 IS 12 AR 121112(R) DI 10.1103/PhysRevB.91.121112 PG 5 WC Physics, Condensed Matter SC Physics GA CE5LG UT WOS:000351875800001 ER PT J AU Schunck, N Duke, D Carr, H AF Schunck, N. Duke, D. Carr, H. TI Description of induced nuclear fission with Skyrme energy functionals. II. Finite temperature effects SO PHYSICAL REVIEW C LA English DT Article ID SELF-CONSISTENT CALCULATIONS; HARMONIC-OSCILLATOR BASIS; HIGHLY EXCITED NUCLEI; HARTREE-FOCK; HOT NUCLEI; ANGULAR-MOMENTUM; MEAN-FIELD; EXCITATION-ENERGY; SHAPE TRANSITIONS; EFFECTIVE FORCES AB Understanding the mechanisms of induced nuclear fission for a broad range of neutron energies could help resolve fundamental science issues, such as the formation of elements in the universe, but could have also a large impact on societal applications in energy production or nuclear waste management. The goal of this paper is to set up the foundations of a microscopic theory to study the static aspects of induced fission as a function of the excitation energy of the incident neutron, from thermal to fast neutrons. To account for the high excitation energy of the compound nucleus, we employ a statistical approach based on finite temperature nuclear density functional theory with Skyrme energy densities, which we benchmark on the Pu-239(n, f) reaction. We compute the evolution of the least-energy fission pathway across multidimensional potential energy surfaces with up to five collective variables as a function of the nuclear temperature and predict the evolution of both the inner and the outer fission barriers as a function of the excitation energy of the compound nucleus. We show that the coupling to the continuum induced by the finite temperature is negligible in the range of neutron energies relevant for many applications of neutron-induced fission. We prove that the concept of quantum localization introduced recently can be extended to T > 0, and we apply the method to study the interaction energy and total kinetic energy of fission fragments as a function of the temperature for the most probable fission. While large uncertainties in theoretical modeling remain, we conclude that a finite temperature nuclear density functional may provide a useful framework to obtain accurate predictions of fission fragment properties. C1 [Schunck, N.] Lawrence Livermore Natl Lab, Div Phys, Livermore, CA 94551 USA. [Duke, D.; Carr, H.] Univ Leeds, Sch Comp, Leeds LS2 9JT, W Yorkshire, England. RP Schunck, N (reprint author), Lawrence Livermore Natl Lab, Div Phys, Livermore, CA 94551 USA. OI Schunck, Nicolas/0000-0002-9203-6849 FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; U.S. Department of Energy Office of Science; Nuclear Physics Program [DE-AC52-07NA27344, Clause B-9999, Clause H-9999]; American Recovery and Reinvestment Act [111-5]; National Center for Computational Sciences (NCCS); National Institute for Computational Sciences (NICS) at Oak Ridge National Laboratory; Livermore Computing Resource Center at Lawrence Livermore National Laboratory; UK Engineering and Physical Sciences Research Council [EP/J013072/1] FX Stimulating discussions with W. Younes, D. Gogny, D. Regnier, and J. Randrup are very gratefully acknowledged. We are also thankful to W. Nazarewicz and J. C. Pei for useful comments. This work was partly performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. Funding was also provided by the U.S. Department of Energy Office of Science, Nuclear Physics Program, pursuant to Contract No. DE-AC52-07NA27344, Clause B-9999, Clause H-9999, and the American Recovery and Reinvestment Act, Pub. L. 111-5. Computational resources were provided through an INCITE grant, "Computational Nuclear Structure," by the National Center for Computational Sciences (NCCS) and National Institute for Computational Sciences (NICS) at Oak Ridge National Laboratory. Additional computing support was provided by the Livermore Computing Resource Center at Lawrence Livermore National Laboratory. Thanks are also due to the UK Engineering and Physical Sciences Research Council, under Grant No. EP/J013072/1. NR 75 TC 8 Z9 8 U1 2 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD MAR 25 PY 2015 VL 91 IS 3 AR 034327 DI 10.1103/PhysRevC.91.034327 PG 17 WC Physics, Nuclear SC Physics GA CE5LH UT WOS:000351876100001 ER PT J AU Lees, JP Poireau, V Tisserand, V Grauges, E Palano, A Eigen, G Stugu, B Brown, DN Kerth, LT Kolomensky, YG Lee, MJ Lynch, G Koch, H Schroeder, T Hearty, C Mattison, TS McKenna, JA So, RY Khan, A Blinov, VE Buzykaev, AR Druzhinin, VP Golubev, VB Kravchenko, EA Onuchin, AP Serednyakov, SI Skovpen, YI Solodov, EP Todyshev, KY Lankford, AJ Dey, B Gary, JW Long, O Sevilla, MF Hong, TM Kovalskyi, D Richman, JD West, CA Eisner, AM Lockman, WS Vazquez, WP Schumm, BA Seiden, A Chao, DS Cheng, CH Echenard, B Flood, KT Hitlin, DG Miyashita, TS Ongmongkolkul, P Porter, FC Rohrken, M Andreassen, R Huard, Z Meadows, BT Pushpawela, BG Sokoloff, MD Sun, L Bloom, PC Ford, WT Gaz, A Smith, G Wagner, SR Ayad, R Toki, WH Spaan, B Bernard, D Verderi, M Playfer, S Bettoni, D Bozzi, C Calabrese, R Cibinetto, G Fioravanti, E Garzia, I Luppi, E Piemontese, L Santoro, V Calcaterra, A De Sangro, R Finocchiaro, G Martellotti, S Patteri, P Peruzzi, IM Piccolo, M Rama, M Zallo, A Contri, R Monge, MR Passaggio, S Patrignani, C Bhuyan, B Prasad, V Adametz, A Uwer, U Lacker, HM Mallik, U Chen, C Cochran, J Prell, S Ahmed, H Gritsan, AV Arnaud, N Davier, M Derkach, D Grosdidier, G Le Diberder, F Lutz, AM Malaescu, B Roudeau, P Stocchi, A Wormser, G Lange, DJ Wright, DM Coleman, JP Fry, JR Gabathuler, E Hutchcroft, DE Payne, DJ Touramanis, C Bevan, AJ Di Lodovico, F Sacco, R Cowan, G Brown, DN Davis, CL Denig, AG Fritsch, M Gradl, W Griessinger, K Hafner, A Schubert, KR Barlow, RJ Lafferty, GD Cenci, R Hamilton, B Jawahery, A Roberts, DA Cowan, R Cheaib, R Patel, PM Robertson, SH Neri, N Palombo, F Cremaldi, L Godang, R Summers, DJ Simard, M Taras, P De Nardo, G Onorato, G Sciacca, C Raven, G Jessop, CP LoSecco, JM Honscheid, K Kass, R Margoni, M Morandin, M Posocco, M Rotondo, M Simi, G Simonetto, F Stroili, R Akar, S Ben-Haim, E Bomben, M Bonneaud, GR Briand, H Calderini, G Chauveau, J Leruste, P Marchiori, G Ocariz, J Biasini, M Manoni, E Rossi, A Angelini, C Batignani, G Bettarini, S Carpinelli, M Casarosa, G Chrzaszcz, M Forti, F Giorgi, MA Lusiani, A Oberhof, B Paoloni, E Rizzo, G Walsh, JJ Pegna, DL Olsen, J Smith, AJS Anulli, F Faccini, R Ferrarotto, F Ferroni, F Gaspero, M Pilloni, A Piredda, G Bunger, C Dittrich, S Grunberg, O Hess, M Leddig, T Voss, C Waldi, R Adye, T Olaiya, EO Wilson, FF Emery, S Vasseur, G Aston, D Bard, DJ Cartaro, C Convery, MR Dorfan, J Dubois-Felsmann, GP Dunwoodie, W Ebert, M Field, RC Fulsom, BG Graham, MT Hast, C Innes, WR Kim, P Leith, DWGS Lindemann, D Luitz, S Luth, V Lynch, HL MacFarlane, DB Muller, DR Neal, H Perl, M Pulliam, T Ratcliff, BN Roodman, A Schindler, RH Snyder, A Su, D Sullivan, MK Va'vra, J Wisniewski, WJ Wulsin, HW Purohit, MV Wilson, JR Randle-Conde, A Sekula, SJ Bellis, M Burchat, PR Puccio, EMT Alam, MS Ernst, JA Gorodeisky, R Guttman, N Peimer, DR Soffer, A Spanier, SM Ritchie, JL Schwitters, RF Izen, JM Lou, XC Bianchi, F De Mori, F Filippi, A Gamba, D Lanceri, L Vitale, L Martinez-Vidal, F Oyanguren, A Villanueva-Perez, P Albert, J Banerjee, S Beaulieu, A Bernlochner, FU Choi, HHF King, GJ Kowalewski, R Lewczuk, MJ Lueck, T Nugent, IM Roney, JM Sobie, RJ Tasneem, N Gershon, TJ Harrison, PF Latham, TE Band, HR Dasu, S Pan, Y Prepost, R Wu, SL AF Lees, J. P. Poireau, V. Tisserand, V. Grauges, E. Palano, A. Eigen, G. Stugu, B. Brown, D. N. Kerth, L. T. Kolomensky, Yu. G. Lee, M. J. Lynch, G. Koch, H. Schroeder, T. Hearty, C. Mattison, T. S. McKenna, J. A. So, R. Y. Khan, A. Blinov, V. E. Buzykaev, A. R. Druzhinin, V. P. Golubev, V. B. Kravchenko, E. A. Onuchin, A. P. Serednyakov, S. I. Skovpen, Yu. I. Solodov, E. P. Todyshev, K. Yu. Lankford, A. J. Dey, B. Gary, J. W. Long, O. Sevilla, M. Franco Hong, T. M. Kovalskyi, D. Richman, J. D. West, C. A. Eisner, A. M. Lockman, W. S. Vazquez, W. Panduro Schumm, B. A. Seiden, A. Chao, D. S. Cheng, C. H. Echenard, B. Flood, K. T. Hitlin, D. G. Miyashita, T. S. Ongmongkolkul, P. Porter, F. C. Rohrken, M. Andreassen, R. Huard, Z. Meadows, B. T. Pushpawela, B. G. Sokoloff, M. D. Sun, L. Bloom, P. C. Ford, W. T. Gaz, A. Smith, G. Wagner, S. R. Ayad, R. Toki, W. H. Spaan, B. Bernard, D. Verderi, M. Playfer, S. Bettoni, D. Bozzi, C. Calabrese, R. Cibinetto, G. Fioravanti, E. Garzia, I. Luppi, E. Piemontese, L. Santoro, V. Calcaterra, A. De Sangro, R. Finocchiaro, G. Martellotti, S. Patteri, P. Peruzzi, I. M. Piccolo, M. Rama, M. Zallo, A. Contri, R. Monge, M. R. Passaggio, S. Patrignani, C. Bhuyan, B. Prasad, V. Adametz, A. Uwer, U. Lacker, H. M. Mallik, U. Chen, C. Cochran, J. Prell, S. Ahmed, H. Gritsan, A. V. Arnaud, N. Davier, M. Derkach, D. Grosdidier, G. Le Diberder, F. Lutz, A. M. Malaescu, B. Roudeau, P. Stocchi, A. Wormser, G. Lange, D. J. Wright, D. M. Coleman, J. P. Fry, J. R. Gabathuler, E. Hutchcroft, D. E. Payne, D. J. Touramanis, C. Bevan, A. J. Di Lodovico, F. Sacco, R. Cowan, G. Brown, D. N. Davis, C. L. Denig, A. G. Fritsch, M. Gradl, W. Griessinger, K. Hafner, A. Schubert, K. R. Barlow, R. J. Lafferty, G. D. Cenci, R. Hamilton, B. Jawahery, A. Roberts, D. A. Cowan, R. Cheaib, R. Patel, P. M. Robertson, S. H. Neri, N. Palombo, F. Cremaldi, L. Godang, R. Summers, D. J. Simard, M. Taras, P. De Nardo, G. Onorato, G. Sciacca, C. Raven, G. Jessop, C. P. LoSecco, J. M. Honscheid, K. Kass, R. Margoni, M. Morandin, M. Posocco, M. Rotondo, M. Simi, G. Simonetto, F. Stroili, R. Akar, S. Ben-Haim, E. Bomben, M. Bonneaud, G. R. Briand, H. Calderini, G. Chauveau, J. Leruste, Ph. Marchiori, G. Ocariz, J. Biasini, M. Manoni, E. Rossi, A. Angelini, C. Batignani, G. Bettarini, S. Carpinelli, M. Casarosa, G. Chrzaszcz, M. Forti, F. Giorgi, M. A. Lusiani, A. Oberhof, B. Paoloni, E. Rizzo, G. Walsh, J. J. Pegna, D. Lopes Olsen, J. Smith, A. J. S. Anulli, F. Faccini, R. Ferrarotto, F. Ferroni, F. Gaspero, M. Pilloni, A. Piredda, G. Bunger, C. Dittrich, S. Grunberg, O. Hess, M. Leddig, T. Voss, C. Waldi, R. Adye, T. Olaiya, E. O. Wilson, F. F. Emery, S. Vasseur, G. Aston, D. Bard, D. J. Cartaro, C. Convery, M. R. Dorfan, J. Dubois-Felsmann, G. P. Dunwoodie, W. Ebert, M. Field, R. C. Fulsom, B. G. Graham, M. T. Hast, C. Innes, W. R. Kim, P. Leith, D. W. G. S. Lindemann, D. Luitz, S. Luth, V. Lynch, H. L. MacFarlane, D. B. Muller, D. R. Neal, H. Perl, M. Pulliam, T. Ratcliff, B. N. Roodman, A. Schindler, R. H. Snyder, A. Su, D. Sullivan, M. K. Va'vra, J. Wisniewski, W. J. Wulsin, H. W. Purohit, M. V. Wilson, J. R. Randle-Conde, A. Sekula, S. J. Bellis, M. Burchat, P. R. Puccio, E. M. T. Alam, M. S. Ernst, J. A. Gorodeisky, R. Guttman, N. Peimer, D. R. Soffer, A. Spanier, S. M. Ritchie, J. L. Schwitters, R. F. Izen, J. M. Lou, X. C. Bianchi, F. De Mori, F. Filippi, A. Gamba, D. Lanceri, L. Vitale, L. Martinez-Vidal, F. Oyanguren, A. Villanueva-Perez, P. Albert, J. Banerjee, Sw. Beaulieu, A. Bernlochner, F. U. Choi, H. H. F. King, G. J. Kowalewski, R. Lewczuk, M. J. Lueck, T. Nugent, I. M. Roney, J. M. Sobie, R. J. Tasneem, N. Gershon, T. J. Harrison, P. F. Latham, T. E. Band, H. R. Dasu, S. Pan, Y. Prepost, R. Wu, S. L. CA BaBar Collaboration TI Measurement of the branching fractions of the radiative leptonic tau decays tau -> e gamma v(v)over-bar and tau -> mu gamma v(v)over-bar at BABAR SO PHYSICAL REVIEW D LA English DT Article ID MONTE-CARLO; DETECTOR AB We perform a measurement of the tau -> l gamma v (v) over bar (l = e, mu) branching fractions for a minimum photon energy of 10 MeV in the tau rest frame, using 431 fb(-1) of e(+) e(-) collisions collected at the center-of-mass energy of the Upsilon(4S) resonance with the BABAR detector at the PEP-II storage rings. We find B(tau -> mu gamma v (v) over bar = (3.69 +/- 0.03 +/- 0.10) x 10(-3) and B(tau -> e gamma v (v) over bar = (1.847 +/- 0.015 +/- 0.052) x 10(-2), where the first quoted error is statistical and the second is systematic. These results are substantially more precise than previous measurements. C1 [Lees, J. P.; Poireau, V.; Tisserand, V.] Univ Savoie, CNRS, IN2P3, LAPP, F-74941 Annecy Le Vieux, France. 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[Bianchi, F.; De Mori, F.; Gamba, D.] Univ Torino, Dipartimento Fis, I-10125 Turin, Italy. [Lanceri, L.; Vitale, L.] Ist Nazl Fis Nucl, Sez Trieste, I-34127 Trieste, Italy. [Lanceri, L.; Vitale, L.] Univ Trieste, Dipartimento Fis, I-34127 Trieste, Italy. [Martinez-Vidal, F.; Oyanguren, A.; Villanueva-Perez, P.] Univ Valencia, CSIC, IFIC, E-46071 Valencia, Spain. [Albert, J.; Banerjee, Sw.; Beaulieu, A.; Bernlochner, F. U.; Choi, H. H. F.; King, G. J.; Kowalewski, R.; Lewczuk, M. J.; Lueck, T.; Nugent, I. M.; Roney, J. M.; Sobie, R. J.; Tasneem, N.] Univ Victoria, Victoria, BC V8W 3P6, Canada. [Gershon, T. J.; Harrison, P. F.; Latham, T. E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Band, H. R.; Dasu, S.; Pan, Y.; Prepost, R.; Wu, S. L.] Univ Wisconsin, Madison, WI 53706 USA. [Carpinelli, M.] Univ Sassari, I-07100 Sassari, Italy. RP Lees, JP (reprint author), Univ Savoie, CNRS, IN2P3, LAPP, F-74941 Annecy Le Vieux, France. RI Calcaterra, Alessandro/P-5260-2015; Lusiani, Alberto/A-3329-2016; Di Lodovico, Francesca/L-9109-2016; Kravchenko, Evgeniy/F-5457-2015; Luppi, Eleonora/A-4902-2015; Calabrese, Roberto/G-4405-2015; Kolomensky, Yury/I-3510-2015; Martinez Vidal, F*/L-7563-2014; Oyanguren, Arantza/K-6454-2014; Monge, Maria Roberta/G-9127-2012; Lusiani, Alberto/N-2976-2015; Forti, Francesco/H-3035-2011; Patrignani, Claudia/C-5223-2009; Morandin, Mauro/A-3308-2016 OI Calcaterra, Alessandro/0000-0003-2670-4826; Lusiani, Alberto/0000-0002-6876-3288; Di Lodovico, Francesca/0000-0003-3952-2175; Luppi, Eleonora/0000-0002-1072-5633; Calabrese, Roberto/0000-0002-1354-5400; Kolomensky, Yury/0000-0001-8496-9975; Martinez Vidal, F*/0000-0001-6841-6035; Oyanguren, Arantza/0000-0002-8240-7300; Monge, Maria Roberta/0000-0003-1633-3195; Lusiani, Alberto/0000-0002-6876-3288; Forti, Francesco/0000-0001-6535-7965; Patrignani, Claudia/0000-0002-5882-1747; Morandin, Mauro/0000-0003-4708-4240 FU US Department of Energy; National Science Foundation; Natural Sciences and Engineering Research Council (Canada); Commissariat a l'Energie Atomique and Institut National de Physique Nucleaire et de Physique des Particules (France); Bundesministerium fur Bildung und Forschung and Deutsche Forschungsgemeinschaft (Germany); Istituto Nazionale di Fisica Nucleare (Italy); Foundation for Fundamental Research on Matter (Netherlands); Research Council of Norway; Ministry of Education and Science of the Russian Federation, Ministerio de Economia y Competitividad (Spain); Science and Technology Facilities Council (United Kingdom); Binational Science Foundation (US-Israel); Marie-Curie IEF program (European Union); A. P. Sloan Foundation (USA) FX We are grateful for the extraordinary contributions of our PEP-II colleagues in achieving the excellent luminosity and machine conditions that have made this work possible. The success of this project also relies critically on the expertise and dedication of the computing organizations that support BABAR. The collaborating institutions wish to thank SLAC for its support and the kind hospitality extended to them. This work is supported by the US Department of Energy and National Science Foundation, the Natural Sciences and Engineering Research Council (Canada), the Commissariat a l'Energie Atomique and Institut National de Physique Nucleaire et de Physique des Particules (France), the Bundesministerium fur Bildung und Forschung and Deutsche Forschungsgemeinschaft (Germany), the Istituto Nazionale di Fisica Nucleare (Italy), the Foundation for Fundamental Research on Matter (Netherlands), the Research Council of Norway, the Ministry of Education and Science of the Russian Federation, Ministerio de Economia y Competitividad (Spain), the Science and Technology Facilities Council (United Kingdom), and the Binational Science Foundation (US-Israel). Individuals have received support from the Marie-Curie IEF program (European Union) and the A. P. Sloan Foundation (USA). NR 19 TC 3 Z9 3 U1 0 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 25 PY 2015 VL 91 IS 5 AR 051103 DI 10.1103/PhysRevD.91.051103 PG 8 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CE5LI UT WOS:000351876200001 ER PT J AU Reichhardt, C Reichhardt, CJO AF Reichhardt, C. Reichhardt, C. J. Olson TI Active microrheology in active matter systems: Mobility, intermittency, and avalanches SO PHYSICAL REVIEW E LA English DT Article ID BROWNIAN PARTICLES AB We examine the mobility and velocity fluctuations of a driven particle moving through an active matter bath of self-mobile disks for varied density or area coverage and varied activity. We show that the driven particle mobility can exhibit nonmonotonic behavior that is correlated with distinct changes in the spatiotemporal structures that arise in the active media. We demonstrate that the probe particle velocity distributions exhibit specific features in the different dynamic regimes and identify an activity-induced uniform crystallization that occurs for moderate activity levels and is distinct from the previously observed higher activity cluster phase. The velocity distribution in the cluster phase has telegraph noise characteristics produced when the probe particle moves alternately through high-mobility areas that are in the gas state and low-mobility areas that are in the dense phase. For higher densities and large activities, the system enters what we characterize as an active jamming regime. Here the probe particle moves in intermittent jumps or avalanches that have power-law-distributed sizes that are similar to the avalanche distributions observed for nonactive disk systems near the jamming transition. C1 [Reichhardt, C.; Reichhardt, C. J. Olson] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Reichhardt, C (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. OI Reichhardt, Cynthia/0000-0002-3487-5089 FU NNSA of the U.S. DOE at LANL [DE-AC52-06NA25396] FX This work was carried out under the auspices of the NNSA of the U.S. DOE at LANL under Contract No. DE-AC52-06NA25396. NR 48 TC 6 Z9 6 U1 2 U2 27 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD MAR 25 PY 2015 VL 91 IS 3 AR 032313 DI 10.1103/PhysRevE.91.032313 PG 7 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA CE5LN UT WOS:000351876900005 PM 25871116 ER PT J AU Salamu, Y Ji, CR Melnitchouk, W Wang, P AF Salamu, Yusupujiang Ji, Chueng-Ryong Melnitchouk, W. Wang, P. TI (d)over-bar - (u)over-bar Asymmetry in the Proton in Chiral Effective Theory SO PHYSICAL REVIEW LETTERS LA English DT Article ID DEEP-INELASTIC-SCATTERING; LIGHT-QUARK SEA; PERTURBATION-THEORY; SYMMETRY-BREAKING; PARTON DISTRIBUTIONS; FLAVOR ASYMMETRY; NUCLEON; SUM AB We compute the (d) over bar - (u) over bar asymmetry in the proton in chiral effective theory, including both nucleon and Delta degrees of freedom, within the relativistic and heavy baryon frameworks. In addition to the distribution at x > 0, we compute the corrections to the asymmetry from zero momentum contributions from pion rainbow and bubble diagrams at x = 0, which have not been accounted for in previous analyses. We find that the empirical x dependence of (d) over bar - (u) over bar as well as the integrated asymmetry can be well reproduced in terms of a transverse momentum cutoff parameter. C1 [Salamu, Yusupujiang; Wang, P.] Chinese Acad Sci, Inst High Energy Phys, Beijing 100049, Peoples R China. [Ji, Chueng-Ryong] N Carolina State Univ, Raleigh, NC 27695 USA. [Melnitchouk, W.] Jefferson Lab, Newport News, VA 23606 USA. [Wang, P.] Chinese Acad Sci, Theoret Phys Ctr Sci Facil, Beijing 100049, Peoples R China. RP Salamu, Y (reprint author), Chinese Acad Sci, Inst High Energy Phys, Beijing 100049, Peoples R China. FU DOE under Jefferson Science Associates, LLC [DE-AC05-06OR23177]; DOE [DE-FG02-03ER41260]; NSFC [11261130311]; DFG [CRC 110]; NSFC FX We are grateful to A. W. Thomas for helpful comments. This work was supported by the DOE Contract No. DE-AC05-06OR23177, under which Jefferson Science Associates, LLC operates Jefferson Lab, DOE Contract No. DE-FG02-03ER41260, and by NSFC under Grant No. 11261130311 (CRC 110 by DFG and NSFC). NR 31 TC 7 Z9 7 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 25 PY 2015 VL 114 IS 12 AR 122001 DI 10.1103/PhysRevLett.114.122001 PG 5 WC Physics, Multidisciplinary SC Physics GA CE5LQ UT WOS:000351877200004 PM 25860735 ER PT J AU Kim, S Petreczky, P Rothkopf, A AF Kim, Seyong Petreczky, Peter Rothkopf, Alexander TI Lattice NRQCD study of S- and P-wave bottomonium states in a thermal medium with N-f=2+1 light flavors SO PHYSICAL REVIEW D LA English DT Article ID QUARK-GLUON PLASMA; NONRELATIVISTIC QCD; SPECTRAL FUNCTIONS; HEAVY QUARKONIUM; HIGH-TEMPERATURE; BOUND-STATES; J/PSI AB We investigate the properties of S- and P-wave bottomonium states in the vicinity of the deconfinement transition temperature. The light degrees of freedom are represented by dynamical lattice quantum chromodynamics (QCD) configurations of the HotQCD collaboration with N-f = 2 + 1 flavors. Bottomonium correlators are obtained from bottom quark propagators, computed in nonrelativistic QCD under the background of these gauge field configurations. The spectral functions for the S-3(1) (Upsilon) and P-3(1) (x(b1)) channel are extracted from the Euclidean time correlators using a novel Bayesian approach in the temperature region 140 MeV <= T <= 249 MeV and the results are contrasted to those from the standard maximum entropy method. We find that the new Bayesian approach is far superior to the maximum entropy method. It enables us to study reliably the presence or absence of the lowest state signal in the spectral function of a certain channel, even under the limitations present in the finite temperature setup. We find that x(b1) survives up to T = 249 MeV, the highest temperature considered in our study, and put stringent constraints on the size of the medium modification of Upsilon and x(b1) states. C1 [Kim, Seyong] Sejong Univ, Dept Phys, Seoul 143747, South Korea. [Petreczky, Peter] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Rothkopf, Alexander] Heidelberg Univ, Inst Theoret Phys, D-69120 Heidelberg, Germany. RP Kim, S (reprint author), Sejong Univ, Dept Phys, Seoul 143747, South Korea. EM skim@sejong.ac.kr FU National Research Foundation of Korea - Korean government (MEST) [2010-002219, NRF-2008000458]; U.S. Department of Energy [DE-AC02-98CH10886]; Swiss National Science Foundation (SNSF) [200021-140234] FX A. R. thanks Y. Burnier for many fruitful discussions. S. K. is supported by the National Research Foundation of Korea funded by the Korean government (MEST) Grant No. 2010-002219 and in part by Grant No. NRF-2008000458. P. P. is supported by the U.S. Department of Energy under Award No. DE-AC02-98CH10886. A. R. was partly supported by the Swiss National Science Foundation (SNSF) under Grant No. 200021-140234. NR 44 TC 7 Z9 7 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 25 PY 2015 VL 91 IS 5 DI 10.1103/PhysRevD.91.054511 PG 28 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CE5LI UT WOS:000351876200009 ER PT J AU Huang, CC Wang, S Pan, LD Barois, P Pindak, R AF Huang, C. C. Wang, Shun Pan, Lidong Barois, P. Pindak, Ron TI Discovery of Liquid Crystal Mesophases with a Six-Layer Periodicity SO MOLECULAR CRYSTALS AND LIQUID CRYSTALS LA English DT Article; Proceedings Paper CT 25th International Liquid Crystal Conference CY JUN 29-JUL 04, 2014 CL Dublin, IRELAND SP Failte Ireland - Nat Tourism Dev Authority DE SmC(*)variant phases; resonant x-ray diffraction; null transmission ellipsometry; SmCd6* phase ID SMECTIC-C TRANSITION; X-RAY-SCATTERING; ALPHA-ASTERISK PHASE; MEAN-FIELD; POLARIZATION; BEHAVIOR; DOBAMBC AB In 2006, employing ellipsometry and resonant x-ray diffraction, our research group discovered a liquid crystal mesophase having a six-layer periodicity in a ternary mixture (mixture A) as well as in a binary mixture (mixture B). This phase shows antiferroelectric-like properties. Subsequently, J. K. Vij's group used field-induced birefringence to explore the physical properties of various binary mixtures similar to mixture B. Recently, Y. Takanishi etal. obtained dielectric responses and two-dimensional microbeam resonant x-ray diffraction profiles as a function of temperature from a different binary mixture with one compound of the mixture containing a central bromine atom. They discovered another new mesophase which shows a six-layer structure and displays ferrielectric-like responses along with a different phase sequence. This article will review the sequence of events leading up to the discovery of the new phases with a six-layer periodicity and highlight differences in conclusions about the new phases and an ongoing debate about the existence of a phase with five-layer periodicity. C1 [Huang, C. C.; Pan, Lidong] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Wang, Shun] Shanghai Jiao Tong Univ, Dept Phys & Astron, Key Lab Artificial Struct & Quantum Control, Minist Educ, Shanghai 200030, Peoples R China. [Pan, Lidong] Johns Hopkins Univ, Dept Phys & Astron, Baltimore, MD USA. [Barois, P.] Univ Bordeaux, CNRS, CRPP, Pessac, France. [Pindak, Ron] Brookhaven Natl Lab, Photon Sci Directorate, Upton, NY 11973 USA. RP Huang, CC (reprint author), Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. EM cchuang@gmail.com RI Shun, Wang/O-6978-2015 OI Shun, Wang/0000-0002-7996-8887 NR 33 TC 0 Z9 0 U1 1 U2 2 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 2-4 PARK SQUARE, MILTON PARK, ABINGDON OR14 4RN, OXON, ENGLAND SN 1542-1406 EI 1563-5287 J9 MOL CRYST LIQ CRYST JI Mol. Cryst. Liquid Cryst. PD MAR 24 PY 2015 VL 610 IS 1 SI SI BP 23 EP 34 DI 10.1080/15421406.2015.1025200 PG 12 WC Crystallography SC Crystallography GA CM1BN UT WOS:000357414800002 ER PT J AU Adam, J Adamova, D Aggarwal, MM Rinella, GA Agnello, M Agrawal, N Ahammed, Z Ahmed, I Ahn, SU Aimo, I Aiola, S Ajaz, M Akindinov, A Alam, SN Aleksandrov, D Alessandro, B Alexandre, D Molina, RA Alici, A Alkin, A Alme, J Alt, T Altinpinar, S Altsybeev, I Prado, CAG Andrei, C Andronic, A Anguelov, V Anielski, J Anticic, T Antinori, F Antonioli, P Aphecetche, L Appelshauser, H Arcelli, S Armesto, N Arnaldi, R Aronsson, T Arsene, IC Arslandok, M Augustinus, A Averbeck, R Azmi, MD Bach, M Badala, A Baek, YW Bagnasco, S Bailhache, R Bala, R Baldisseri, A Ball, M Pedrosa, FBD Baral, RC Barbano, AM Barbera, R Barile, F Barnafoldi, GG Barnby, LS Barret, V Bartalini, P Bartke, J Bartsch, E Basile, M Bastid, N Basu, S Bathen, B Batigne, G Camejo, AB Batyunya, B Batzing, PC Bearden, IG Beck, H Bedda, C Behera, NK Belikov, I Bellini, F Martinez, HB Bellwied, R Belmont, R Belmont-Moreno, E Belyaev, V Bencedi, G Beole, S Berceanu, I Bercuci, A Berdnikov, Y Berenyi, D Bertens, RA Berzano, D Betev, L Bhasin, A Bhat, IR Bhati, AK Bhattacharjee, B Bhom, J Bianchi, L Bianchi, N Bianchin, C Bielcik, J Bielcikova, J Bilandzic, A Biswas, S Bjelogrlic, S Blanco, F Blau, D Blume, C Bock, F Bogdanov, A Boggild, H Boldizsar, L Bombara, M Book, J Borel, H Borissov, A Borri, M Bossu, F Botje, M Botta, E Bottger, S Braun-Munzinger, P Bregant, M Breitner, T Broker, TA Browning, TA Broz, M Brucken, EJ Bruna, E Bruno, GE Budnikov, D Buesching, H Bufalino, S Buncic, P Busch, O Buthelezi, Z Buxton, JT Caffarri, D Cai, X Caines, H Diaz, LC Caliva, A Villar, EC Camerini, P Carena, F Carena, W Castellanos, JC Castro, AJ Casula, EAR Cavicchioli, C Sanchez, CC Cepila, J Cerello, P Chang, B Chapeland, S Chartier, M Charvet, JL Chattopadhyay, S Chattopadhyay, S Chelnokov, V Cherney, M Cheshkov, C Cheynis, B Barroso, VC Chinellato, DD Chochula, P Choi, K Chojnacki, M Choudhury, S Christakoglou, P Christensen, CH Christiansen, P Chujo, T Chung, SU Cicalo, C Cifarelli, L Cindolo, F Cleymans, J Colamaria, F Colella, D Collu, A Colocci, M Balbastre, GC del Valle, ZC Connors, ME Contreras, JG Cormier, TM Morales, YC Maldonado, IC Cortese, P Cosentino, MR Costa, F Crochet, P Albino, RC Cuautle, E Cunqueiro, L Dahms, T Dainese, A Danu, A Das, D Das, I Das, S Dash, A Dash, S De, S De Caro, A de Cataldo, G de Cuveland, J De Falco, A De Gruttola, D De Marco, N De Pasquale, S Deisting, A Deloff, A Denes, E D'Erasmo, G Di Bari, D Di Mauro, A Di Nezza, P Corchero, MAD Dietel, T Dillenseger, P Divia, R Djuvsland, O Dobrin, A Dobrowolski, T Gimenez, DD Donigus, B Dordic, O Dubey, AK Dubla, A Ducroux, L Dupieux, P Ehlers, RJ Elia, D Engel, H Erazmus, B Erhardt, F Eschweiler, D Espagnon, B Estienne, M Esumi, S Evans, D Evdokimov, S Eyyubova, G Fabbietti, L Fabris, D Faivre, J Fantoni, A Fasel, M Feldkamp, L Felea, D Feliciello, A Feofilov, G Ferencei, J Tellez, AF Ferreiro, EG Ferretti, A Festanti, A Figiel, J Figueredo, MAS Filchagin, S Finogeev, D Fionda, FM Fiore, EM Floris, M Foertsch, S Foka, P Fokin, S Fragiacomo, E Francescon, A Frankenfeld, U Fuchs, U Furget, C Furs, A Girard, MF Gaardhoje, JJ Gagliardi, M Gago, AM Gallio, M Gangadharan, DR Ganoti, P Gao, C Garabatos, C Garcia-Solis, E Gargiulo, C Gasik, P Germain, M Gheata, A Gheata, M Ghosh, P Ghosh, SK Gianotti, P Giubellino, P Giubilato, P Gladysz-Dziadus, E Glassel, P Ramirez, AG Gonzalez-Zamora, P Gorbunov, S Gorlich, L Gotovac, S Grabski, V Graczykowski, LK Grelli, A Grigoras, A Grigoras, C Grigoriev, V Grigoryan, A Grigoryan, S Grinyov, B Grion, N Grosse-Oetringhaus, JF Grossiord, JY Grosso, R Guber, F Guernane, R Guerzoni, B Gulbrandsen, K Gulkanyan, H Gunji, T Gupta, A Gupta, R Haake, R Haaland, O Hadjidakis, C Haiduc, M Hamagaki, H Hamar, G Hanratty, LD Hansen, A Harris, JW Hartmann, H Harton, A Hatzifotiadou, D Hayashi, S Heckel, ST Heide, M Helstrup, H Herghelegiu, A Corral, GH Hess, BA Hetland, KF Hilden, TE Hillemanns, H Hippolyte, B Hristov, P Huang, M Humanic, TJ Hussain, N Hussain, T Hutter, D Hwang, DS Ilkaev, R Ilkiv, I Inaba, M Ionita, C Ippolitov, M Irfan, M Ivanov, M Ivanov, V Izucheev, V Jacobs, PM Jahnke, C Jang, HJ Janik, MA Jayarathna, PHSY Jena, C Jena, S Bustamante, RTJ Jones, PG Jung, H Jusko, A Kadyshevskiy, V Kalinak, P Kalweit, A Kamin, J Kang, JH Kaplin, V Kar, S Uysal, AK Karavichev, O Karavicheva, T Karpechev, E Kebschull, U Keidel, R Keijdener, DLD Keil, M Khan, KH Khan, MM Khan, P Khan, SA Khanzadeev, A Kharlov, Y Kileng, B Kim, B Kim, DW Kim, DJ Kim, H Kim, JS Kim, M Kim, M Kim, S Kim, T Kirsch, S Kisel, I Kiselev, S Kisiel, A Kiss, G Klay, JL Klein, C Klein, J Klein-Bosing, C Kluge, A Knichel, ML Knospe, AG Kobayashi, T Kobdaj, C Kofarago, M Kohler, MK Kollegger, T Kolojvari, A Kondratiev, V Kondratyeva, N Kondratyuk, E Konevskikh, A Kouzinopoulos, C Kovalenko, V Kowalski, M Kox, S Meethaleveedu, GK Kral, J Kralik, I Kravcakova, A Krelina, M Kretz, M Krivda, M Krizek, F Kryshen, E Krzewicki, M Kubera, AM Kucera, V Kucheriaev, Y Kugathasan, T Kuhn, C Kuijer, PG Kulakov, I Kumar, J Kurashvili, P Kurepin, A Kurepin, AB Kuryakin, A Kushpil, S Kweon, MJ Kwon, Y La Pointe, SL La Rocca, P Fernandes, CL Lakomov, I Langoy, R Lara, C Lardeux, A Lattuca, A Laudi, E Lea, R Leardini, L Lee, GR Lee, S Legrand, I Lehnert, J Lemmon, RC Lenti, V Leogrande, E Monon, IL Leoncino, M Levai, P Li, S Li, X Lien, J Lietava, R Lindal, S Lindenstruth, V Lippmann, C Lisa, MA Ljunggren, HM Lodato, DF Loenne, PI Loggins, VR Loginov, V Loizides, C Lokesh, K Lopez, X Torres, EL Lowe, A Lu, XG Luettig, P Lunardon, M Luparello, G Maevskaya, A Mager, M Mahajan, S Mahmood, SM Maire, A Majka, RD Malaev, M Cervantes, IM Malinina, L Mal'Kevich, D Malzacher, P Mamonov, A Manceau, L Manko, V Manso, F Manzari, V Marchisone, M Mares, J Margagliotti, GV Margotti, A Margutti, J Marin, A Markert, C Marquard, M Martashvili, I Martin, NA Blanco, JM Martinengo, P Martinez, MI Garcia, GM Pedreira, MM Martynov, Y Mas, A Masciocchi, S Masera, M Masoni, A Massacrier, L Mastroserio, A Matyja, A Mayer, C Mazer, J Mazzoni, MA Mcdonald, D Meddi, F Menchaca-Rocha, A Meninno, E Perez, JM Meres, M Miake, Y Mieskolainen, MM Mikhaylov, K Milano, L Milosevic, J Minervini, LM Mischke, A Mishra, AN Miskowiec, D Mitra, J Mitu, CM Mohammadi, N Mohanty, B Molnar, L Zetina, LM Montes, E Morando, M De Godoy, DAM Moretto, S Morreale, A Morsch, A Muccifora, V Mudnic, E Muhlheim, D Muhuri, S Mukherjee, M Muller, H Mulligan, JD Munhoz, MG Murray, S Musa, L Musinsky, J Nandi, BK Nania, R Nappi, E Naru, MU Nattrass, C Nayak, K Nayak, TK Nazarenko, S Nedosekin, A Nellen, L Ng, F Nicassio, M Niculescu, M Niedziela, J Nielsen, BS Nikolaev, S Nikulin, S Nikulin, V Noferini, F Nomokonov, P Nooren, G Norman, J Nyanin, A Nystrand, J Oeschler, H Oh, S Oh, SK Ohlson, A Okatan, A Okubo, T Olah, L Oleniacz, J Da Silva, ACO Oliver, MH Onderwaater, J 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Watanabe, D. Weber, M. Weber, S. G. Wessels, J. P. Westerhoff, U. Wiechula, J. Wikne, J. Wilde, M. Wilk, G. Wilkinson, J. Williams, M. C. S. Windelband, B. Winn, M. Yaldo, C. G. Yamaguchi, Y. Yang, H. Yang, P. Yano, S. Yasnopolskiy, S. Yin, Z. Yokoyama, H. Yoo, I. -K. Yurchenko, V. Yushmanov, I. Zaborowska, A. Zaccolo, V. Zaman, A. Zampolli, C. Zanoli, H. J. C. Zaporozhets, S. Zarochentsev, A. Zavada, P. Zaviyalov, N. Zbroszczyk, H. Zgura, I. S. Zhalov, M. Zhang, H. Zhang, X. Zhang, Y. Zhao, C. Zhigareva, N. Zhou, D. Zhou, Y. Zhou, Z. Zhu, H. Zhu, J. Zhu, X. Zichichi, A. Zimmermann, A. Zimmermann, M. B. Zinovjev, G. Zyzak, M. TI Two-pion femtoscopy in p-Pb collisions at root(NN)-N-S=5.02 TeV SO PHYSICAL REVIEW C LA English DT Article ID CHARGED-PARTICLE PRODUCTION; BOSE-EINSTEIN CORRELATIONS; LARGE TRANSVERSE-MOMENTUM; QUARK-GLUON PLASMA; ROOT-S(NN)=2.76 TEV; CENTRALITY DEPENDENCE; COULOMB CORRECTIONS; EMISSION SOURCE; COLLABORATION; PERSPECTIVE AB We report the results of the femtoscopic analysis of pairs of identical pions measured in p-Pb collisions at root(NN)-N-S = 5.02 TeV. Femtoscopic radii are determined as a function of event multiplicity and pair momentum in three spatial dimensions. As in the pp collision system, the analysis is complicated by the presence of sizable background correlation structures in addition to the femtoscopic signal. The radii increase with event multiplicity and decrease with pair transverse momentum. When taken at comparable multiplicity, the radii measured in p-Pb collisions, at high multiplicity and low pair transverse momentum, are 10%-20% higher than those observed in pp collisions but below those observed in A-A collisions. The results are compared to hydrodynamic predictions at large event multiplicity as well as discussed in the context of calculations based on gluon saturation. C1 [Grigoryan, A.; Gulkanyan, H.; Papikyan, V.] Yerevan Phys Inst Fdn, AI Alikhanyan Natl Sci Lab, Yerevan, Armenia. [Martinez, H. Bello; Maldonado, I. Cortes; Tellez, A. Fernandez; Martinez, M. I.; Cahuantzi, M. Rodriguez; Munoz, G. Tejeda; Vargas, A.; Limon, S. Vergara] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Alkin, A.; Chelnokov, V.; Grinyov, B.; Martynov, Y.; Shadura, O.; Trubnikov, V.; Yurchenko, V.] Bogolyubov Inst Theoret Phys, Kiev, Ukraine. [Das, S.; Ghosh, S. K.; Prasad, S. K.; Raha, S.] Bose Inst, Dept Phys, Kolkata, India. [Das, S.; Ghosh, S. K.; Prasad, S. 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Martinez; Massacrier, L.; De Godoy, D. A. Moreira; Morreale, A.; Pillot, P.; Ronflette, L.; Schutz, Y.; Shabetai, A.; Suleymanov, M.; Wang, M.; Zhu, J.] Univ Nantes, Ecole Mines Nantes, SUBATECH, CNRS IN2P3, Nantes, France. [Kobdaj, C.] Suranaree Univ Technol, Nakhon Ratchasima, Thailand. [Gotovac, S.; Mudnic, E.; Vickovic, L.] Tech Univ Split FESB, Split, Croatia. [Bartke, J.; Figiel, J.; Gladysz-Dziadus, E.; Goerlich, L.; Kowalski, M.; Matyja, A.; Mayer, C.; Otwinowski, J.; Rybicki, A.; Sputowska, I.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Knospe, A. G.; Markert, C.; Thomas, D.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Monzon, I. Leon; Podesta-Lerma, P. L. M.] Univ Autonoma Sinaloa, Culiacan, Mexico. [Prado, C. Alves Garcia; Bregant, M.; Cosentino, M. R.; De, S.; Gimenez, D. Domenicis; Jahnke, C.; Fernandes, C. Lagana; Mas, A.; Munhoz, M. G.; Da Silva, A. C. Oliveira; De Oliveira Filho, E. Pereira; Seeder, K. 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[Bhom, J.; Chujo, T.; Esumi, S.; Inaba, M.; Kobayashi, T.; Miake, Y.; Sano, M.; Tanaka, N.; Watanabe, D.; Yokoyama, H.] Univ Tsukuba, Tsukuba, Ibaraki, Japan. [Erhardt, F.; Planinic, M.; Poljak, N.; Simatovic, G.; Utrobicic, A.] Univ Zagreb, Zagreb 41000, Croatia. [Cheshkov, C.; Cheynis, B.; Ducroux, L.; Grossiord, J. -Y.; Teyssier, B.; Tieulent, R.; Uras, A.] Univ Lyon 1, Univ Lyon, CNRS IN2P3, IPN Lyon, F-69622 Villeurbanne, France. [Altsybeev, I.; Feofilov, G.; Kolojvari, A.; Kondratiev, V.; Kovalenko, V.; Vechernin, V.; Vinogradov, L.; Zarochentsev, A.] St Petersburg State Univ, V Fock Inst Phys, St Petersburg 199034, Russia. [Ahammed, Z.; Alam, S. N.; Basu, S.; Chattopadhyay, S.; Choudhury, S.; De, S.; Dubey, A. K.; Ghosh, P.; Kar, S.; Khan, S. A.; Mitra, J.; Mohanty, B.; Muhuri, S.; Mukherjee, M.; Nayak, T. K.; Pal, S. K.; Saini, J.; Sarkar, D.; Singaraju, R.; Singha, S.; Singhal, V.; Sinha, B. C.; Viyogi, Y. P.] Ctr Variable Energy Cyclotron, Kolkata, India. [Graczykowski, L. K.; Janik, M. A.; Kisiel, A.; Oleniacz, J.; Pawlak, T.; Pluta, J.; Szymanski, M.; Zaborowska, A.; Zbroszczyk, H.] Warsaw Univ Technol, Warsaw, Poland. [Belmont, R.; Bianchin, C.; Loggins, V. R.; Pan, J.; Pruneau, C. A.; Pujahari, P.; Putschke, J.; Reed, R. J.; Saleh, M. A.; Verweij, M.; Voloshin, S. A.; Yaldo, C. G.] Wayne State Univ, Detroit, MI USA. [Bencedi, G.; Berenyi, D.; Denes, E.; Hamar, G.; Kiss, G.; Lowe, A.; Varga, D.; Volpe, G.] Hungarian Acad Sci, Wigner Res Ctr Phys, Budapest, Hungary. [Aiola, S.; Aronsson, T.; Caines, H.; Connors, M. E.; Ehlers, R. J.; Harris, J. W.; Majka, R. D.; Mulligan, J. D.; Oh, S.; Oliver, M. H.; Schuster, T.; Smirnov, N.] Yale Univ, New Haven, CT USA. [Kang, J. H.; Kim, B.; Kim, H.; Kim, M.; Kim, T.; Kwon, Y.; Lee, S.; Song, M.] Yonsei Univ, Seoul 120749, South Korea. [Keidel, R.] ZTT, Fachhochsch Worms, Worms, Germany. [Malinina, L.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Milosevic, J.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Redlich, K.] Univ Wroclaw, Inst Theoret Phys, PL-50138 Wroclaw, Poland. [Takaki, J. D. Tapia] Univ Kansas, Lawrence, KS 66045 USA. RP Adam, J (reprint author), Czech Tech Univ, Fac Nucl Sci & Phys Engn, CR-11519 Prague, Czech Republic. RI Vickovic, Linda/F-3517-2017; Fernandez Tellez, Arturo/E-9700-2017; Cosentino, Mauro/L-2418-2014; Peitzmann, Thomas/K-2206-2012; Suaide, Alexandre/L-6239-2016; Vinogradov, Leonid/K-3047-2013; Castillo Castellanos, Javier/G-8915-2013; Inst. of Physics, Gleb Wataghin/A-9780-2017; Ferreiro, Elena/C-3797-2017; Armesto, Nestor/C-4341-2017; Martinez Hernandez, Mario Ivan/F-4083-2010; Ferretti, Alessandro/F-4856-2013; Adamova, Dagmar/G-9789-2014; Christensen, Christian/D-6461-2012; De Pasquale, Salvatore/B-9165-2008; Chinellato, David/D-3092-2012; Felea, Daniel/C-1885-2012; de Cuveland, Jan/H-6454-2016; Kurepin, Alexey/H-4852-2013; Jena, Deepika/P-2873-2015; Akindinov, Alexander/J-2674-2016; Takahashi, Jun/B-2946-2012; Nattrass, Christine/J-6752-2016; Usai, Gianluca/E-9604-2015; Pshenichnov, Igor/A-4063-2008; Guber, Fedor/I-4271-2013; Zarochentsev, Andrey/J-6253-2013; Altsybeev, Igor/K-6687-2013; Kondratiev, Valery/J-8574-2013; Vechernin, Vladimir/J-5832-2013; Naru, Muhammad Umair/N-5547-2015; Janik, Malgorzata/O-7520-2015; Graczykowski, Lukasz/O-7522-2015; Sevcenco, Adrian/C-1832-2012; feofilov, grigory/A-2549-2013; HAMAGAKI, HIDEKI/G-4899-2014; Kovalenko, Vladimir/C-5709-2013; Salgado, Carlos A./G-2168-2015; Bregant, Marco/I-7663-2012; Kucera, Vit/G-8459-2014; Krizek, Filip/G-8967-2014; Bielcikova, Jana/G-9342-2014; Vajzer, Michal/G-8469-2014; Sumbera, Michal/O-7497-2014; Barnby, Lee/G-2135-2010; Barbera, Roberto/G-5805-2012; Bruna, Elena/C-4939-2014; Karasu Uysal, Ayben/K-3981-2015 OI Vickovic, Linda/0000-0002-9820-7960; Fernandez Tellez, Arturo/0000-0003-0152-4220; Riggi, Francesco/0000-0002-0030-8377; Scarlassara, Fernando/0000-0002-4663-8216; Giubilato, Piero/0000-0003-4358-5355; Fernandez Tellez, Arturo/0000-0001-5092-9748; Cosentino, Mauro/0000-0002-7880-8611; Peitzmann, Thomas/0000-0002-7116-899X; Suaide, Alexandre/0000-0003-2847-6556; Vinogradov, Leonid/0000-0001-9247-6230; Castillo Castellanos, Javier/0000-0002-5187-2779; Ferreiro, Elena/0000-0002-4449-2356; Armesto, Nestor/0000-0003-0940-0783; Martinez Hernandez, Mario Ivan/0000-0002-8503-3009; Ferretti, Alessandro/0000-0001-9084-5784; Christensen, Christian/0000-0002-1850-0121; De Pasquale, Salvatore/0000-0001-9236-0748; Chinellato, David/0000-0002-9982-9577; Felea, Daniel/0000-0002-3734-9439; de Cuveland, Jan/0000-0003-0455-1398; Kurepin, Alexey/0000-0002-1851-4136; Jena, Deepika/0000-0003-2112-0311; Akindinov, Alexander/0000-0002-7388-3022; Takahashi, Jun/0000-0002-4091-1779; Nattrass, Christine/0000-0002-8768-6468; Usai, Gianluca/0000-0002-8659-8378; Pshenichnov, Igor/0000-0003-1752-4524; Guber, Fedor/0000-0001-8790-3218; Zarochentsev, Andrey/0000-0002-3502-8084; Altsybeev, Igor/0000-0002-8079-7026; Kondratiev, Valery/0000-0002-0031-0741; Vechernin, Vladimir/0000-0003-1458-8055; Naru, Muhammad Umair/0000-0001-6489-0784; Janik, Malgorzata/0000-0002-3356-3438; Sevcenco, Adrian/0000-0002-4151-1056; feofilov, grigory/0000-0003-3700-8623; Kovalenko, Vladimir/0000-0001-6012-6615; Salgado, Carlos A./0000-0003-4586-2758; Sumbera, Michal/0000-0002-0639-7323; Barnby, Lee/0000-0001-7357-9904; Barbera, Roberto/0000-0001-5971-6415; Bruna, Elena/0000-0001-5427-1461; Karasu Uysal, Ayben/0000-0001-6297-2532 FU Worldwide LHC Computing Grid (WLCG) collaboration; State Committee of Science; World Federation of Scientists (WFS); Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq); Financiadora de Estudos e Projetos (FINEP); Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC); Chinese Ministry of Education (CMOE); Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council; Carlsberg Foundation; Danish National Research Foundation; European Research Council under the European Community's Seventh Framework Programme; Helsinki Institute of Physics; Academy of Finland; French CNRS-IN2P3, France; Region Pays de Loire, France; Region Alsace, France; Region Auvergne, France; CEA, France; German Bundesministerium fur Bildung, Wissenschaft, Forschung und Technologie (BMBF); Helmholtz Association; General Secretariat for Research and Technology, Greece; Ministry of Development, Greece; Hungarian Orszagos Tudomanyos Kutatasi Alappgrammok (OTKA); National Office for Research and Technology (NKTH); Department of Atomic Energy; Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN); Centro Fermi-Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi," Italy; MEXT, Japan; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); Consejo Nacional de Cienca y Tecnologia (CONACYT), Mexico; Direccion General de Asuntos del Personal Academico (DGAPA), Mexico; Amerique Latine Formation academique European Commission (ALFA-EC); EPLANET Program (European Particle Physics Latin American Network); Stichting voor Fundamenteel Onderzoek der Materie (FOM), Netherlands; Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); National Science Centre, Poland; Ministry of National Education/Institute for Atomic Physics; Consiliul National al Cercetrii ztiinifice-Executive Agency for Higher Education Research Development and Innovation Funding (CNCS-UEFISCDI)-Romania; Ministry of Education and Science of Russian Federation; Russian Academy of Sciences; Russian Federal Agency of Atomic Energy; Russian Federal Agency for Science and Innovations; Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, South Africa; Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas (CIEMAT); E-Infrastructure shared between Europe and Latin America (EELA); Ministerio de Economia y Competitividad (MINECO) of Spain; Xunta de Galicia (Conselleria de Educacion); Centro de Aplicaciones Tecnolgicas y Desarrollo Nuclear (CEADEN), Cuba; IAEA (International Atomic Energy Agency); Swedish Research Council (VR); Knut AMP; Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); United States Department of Energy; United States National Science Foundation; State of Texas; State of Ohio; Ministry of Science, Education and Sports of Croatia, Croatia; Unity through Knowledge Fund, Croatia; Council of Scientific and Industrial Research (CSIR), New Delhi, India; Cubaenergia, Cuba FX The ALICE Collaboration would like to thank all its engineers and technicians for their invaluable contributions to the construction of the experiment and the CERN accelerator teams for the outstanding performance of the LHC complex. The ALICE Collaboration gratefully acknowledges the resources and support provided by all Grid centers and the Worldwide LHC Computing Grid (WLCG) collaboration.; r The ALICE Collaboration acknowledges the following funding agencies for their support in building and running the ALICE detector: State Committee of Science, World Federation of Scientists (WFS) and Swiss Fonds Kidagan, Armenia, Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq), Financiadora de Estudos e Projetos (FINEP), Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC), the Chinese Ministry of Education (CMOE) and the Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council, the Carlsberg Foundation and the Danish National Research Foundation; The European Research Council under the European Community's Seventh Framework Programme; Helsinki Institute of Physics and the Academy of Finland; French CNRS-IN2P3, the "Region Pays de Loire," "Region Alsace," "Region Auvergne" and CEA, France; German Bundesministerium fur Bildung, Wissenschaft, Forschung und Technologie (BMBF) and the Helmholtz Association; General Secretariat for Research and Technology, Ministry of Development, Greece; Hungarian Orszagos Tudomanyos Kutatasi Alappgrammok (OTKA) and National Office for Research and Technology (NKTH); Department of Atomic Energy and Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN) and Centro Fermi-Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi," Italy; MEXT Grant-in-Aid for Specially Promoted Research, Japan; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); Consejo Nacional de Cienca y Tecnologia (CONACYT), Direccion General de Asuntos del Personal Academico (DGAPA), Mexico; Amerique Latine Formation academique European Commission (ALFA-EC) and the EPLANET Program (European Particle Physics Latin American Network); Stichting voor Fundamenteel Onderzoek der Materie (FOM) and the Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); National Science Centre, Poland; Ministry of National Education/Institute for Atomic Physics and Consiliul National al Cercetrii ztiinifice-Executive Agency for Higher Education Research Development and Innovation Funding (CNCS-UEFISCDI)-Romania; Ministry of Education and Science of Russian Federation, Russian Academy of Sciences, Russian Federal Agency of Atomic Energy, Russian Federal Agency for Science and Innovations and The Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, South Africa; Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas (CIEMAT), E-Infrastructure shared between Europe and Latin America (EELA); Ministerio de Economia y Competitividad (MINECO) of Spain; Xunta de Galicia (Conselleria de Educacion), Centro de Aplicaciones Tecnolgicas y Desarrollo Nuclear (CEADEN), Cubaenergia, Cuba; and IAEA (International Atomic Energy Agency); Swedish Research Council (VR) and Knut & Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); The United States Department of Energy, the United States National Science Foundation, the State of Texas, and the State of Ohio; Ministry of Science, Education and Sports of Croatia and Unity through Knowledge Fund, Croatia; Council of Scientific and Industrial Research (CSIR), New Delhi, India NR 54 TC 17 Z9 17 U1 1 U2 76 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD MAR 24 PY 2015 VL 91 IS 3 AR 034906 DI 10.1103/PhysRevC.91.034906 PG 18 WC Physics, Nuclear SC Physics GA CH3EW UT WOS:000353911600006 ER PT J AU Mecca, A Lovato, A Benhar, O Polls, A AF Mecca, Angela Lovato, Alessandro Benhar, Omar Polls, Artur TI Effective-interaction approach to the Fermi hard-sphere system SO PHYSICAL REVIEW C LA English DT Article ID CORRELATED-BASIS THEORY; NUCLEAR-MATTER; MOMENTUM DISTRIBUTION; GAS; ENERGY; SCATTERING; FLUIDS AB The formalism based on correlated basis functions and the cluster-expansion technique has been recently employed to derive an effective interaction from a realistic nuclear Hamiltonian. To gauge the reliability of this scheme, we perform a systematic comparison between the results of its application to the Fermi hard-sphere system and the predictions obtained from low-density expansions, as well as from other many-body techniques. The analysis of a variety of properties, including the ground-state energy, the effective mass, and the momentum distribution, shows that the effective-interaction approach is quite accurate, thus suggesting that it may be employed to achieve a consistent description of the structure and dynamics of nuclear matter in the density region relevant to astrophysical applications. C1 [Mecca, Angela; Benhar, Omar] Ist Nazl Fis Nucl, Sez Roma, I-00185 Rome, Italy. [Mecca, Angela; Benhar, Omar] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Lovato, Alessandro] Argonne Natl Lab, Argonne Leadership Comp Facil, Argonne, IL 60439 USA. [Lovato, Alessandro] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Polls, Artur] Dept Estruct & Constituents Mat, E-08028 Barcelona, Spain. RP Mecca, A (reprint author), Ist Nazl Fis Nucl, Sez Roma, I-00185 Rome, Italy. RI Polls, Artur/K-7643-2014; OI Polls, Artur/0000-0002-3272-106X; Lovato, Alessandro/0000-0002-2194-4954 FU US Department of Energy, Office of Science, Office of Nuclear Physics [DE-AC02-06CH11357]; MICINN (Spain) [FI-2011-24154]; Generalitat de Catalunya [2014SGR-401]; INFN (Italy) [MANYBODY]; COST Action [MP1304]; NewCompStar FX This research is supported by the US Department of Energy, Office of Science, Office of Nuclear Physics, under contract DE-AC02-06CH11357 (AL), MICINN (Spain), under Grant No. FI-2011-24154 and Generalitat de Catalunya, under grant 2014SGR-401 (AP), and INFN (Italy) under Grant No. MANYBODY (AM and OB). AM gratefully acknowledges the hospitality of the Departament d'Estructura i Constituents de la Materia of the University of Barcelona, and support from "NewCompStar," COST Action MP1304. NR 42 TC 3 Z9 3 U1 0 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAR 24 PY 2015 VL 91 IS 3 AR 034325 DI 10.1103/PhysRevC.91.034325 PG 11 WC Physics, Nuclear SC Physics GA CH3EW UT WOS:000353911600002 ER PT J AU Biedermann, GW Wu, X Deslauriers, L Roy, S Mahadeswaraswamy, C Kasevich, MA AF Biedermann, G. W. Wu, X. Deslauriers, L. Roy, S. Mahadeswaraswamy, C. Kasevich, M. A. TI Testing gravity with cold-atom interferometers SO PHYSICAL REVIEW A LA English DT Article ID INVERSE-SQUARE LAW; CONSTANT AB We present a horizontal gravity gradiometer atom interferometer for precision gravitational tests. The horizontal configuration is superior for maximizing the inertial signal in the atom interferometer from a nearby proof mass. In our device, we have suppressed spurious noise associated with the horizonal configuration to achieve a differential acceleration sensitivity of 4.2x10(-9) g/root Hz over a 70-cm baseline or 3.0x10(-9) g/root Hz inferred per accelerometer. Using the performance of this instrument, we characterize the results of possible future gravitational tests. We demonstrate a statistical uncertainty of 3x10(-4) for a proof-of-concept measurement of the gravitational constant that is competitive with the present limit of 1.2x10(-4) using other techniques. From this measurement, we provide a statistical constraint on a Yukawa-type fifth force at 8x10(-3) near the poorly known length scale of 10 cm. Limits approaching 10(-5) appear feasible. We discuss improvements that can enable uncertainties falling well below 10(-5) for both experiments. C1 [Biedermann, G. W.; Wu, X.; Deslauriers, L.; Roy, S.; Mahadeswaraswamy, C.; Kasevich, M. A.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. RP Biedermann, GW (reprint author), Sandia Natl Labs, Albuquerque, NM 87123 USA. EM kasevich@stanford.edu FU AFRL [F19628-02-C-0096]; DARPA [W911NF-06-1-0064] FX We are indebted to Kai Bongs, Matt Cashen, Jeff Fixler, Todd Gustavson, Ken Takase, and Brent Young for countless contributions to the design and construction of the apparatus. This work was supported by AFRL under Contract No. F19628-02-C-0096 and DARPA under Contract No. W911NF-06-1-0064. NR 39 TC 16 Z9 18 U1 8 U2 49 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1050-2947 EI 1094-1622 J9 PHYS REV A JI Phys. Rev. A PD MAR 24 PY 2015 VL 91 IS 3 AR 033629 DI 10.1103/PhysRevA.91.033629 PG 10 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA CH3EA UT WOS:000353908600006 ER PT J AU Marshall, K Pooser, R Siopsis, G Weedbrook, C AF Marshall, Kevin Pooser, Raphael Siopsis, George Weedbrook, Christian TI Repeat-until-success cubic phase gate for universal continuous-variable quantum computation SO PHYSICAL REVIEW A LA English DT Article ID STATES; INFORMATION; EFFICIENCY AB To achieve universal quantum computation using continuous variables, one needs to jump out of the set of Gaussian operations and have a non-Gaussian element, such as the cubic phase gate. However, such a gate is currently very difficult to implement in practice. Here we introduce an experimentally viable "repeat-untilsuccess" approach to generating the cubic phase gate, which is achieved using sequential photon subtractions and Gaussian operations. We find that our scheme offers benefits in terms of the expected time until success, as well as the fact that we do not require any complex off-line resource state, although we require a primitive quantum memory. C1 [Marshall, Kevin] Univ Toronto, Dept Phys, Toronto, ON M5S 1A7, Canada. [Pooser, Raphael] Oak Ridge Natl Lab, Quantum Informat Sci Grp, Oak Ridge, TN 37831 USA. [Pooser, Raphael] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Weedbrook, Christian] QKD Corp, Toronto, ON M5S 1A7, Canada. RP Marshall, K (reprint author), Univ Toronto, Dept Phys, 60 St George St, Toronto, ON M5S 1A7, Canada. OI Pooser, Raphael/0000-0002-2922-453X FU NSERC; US Department of Energy [DE-AC05-00OR22725] FX We are grateful to Radim Filip for useful dialogue. K.M. acknowledges support from NSERC. R.C.P. performed portions of this work at Oak Ridge National Laboratory, operated by UT-Battelle for the US Department of Energy under Contract No. DE-AC05-00OR22725. NR 32 TC 6 Z9 6 U1 0 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1050-2947 EI 1094-1622 J9 PHYS REV A JI Phys. Rev. A PD MAR 24 PY 2015 VL 91 IS 3 AR 032321 DI 10.1103/PhysRevA.91.032321 PG 7 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA CH3EA UT WOS:000353908600004 ER PT J AU McDonnell, JD Schunck, N Higdon, D Sarich, J Wild, SM Nazarewicz, W AF McDonnell, J. D. Schunck, N. Higdon, D. Sarich, J. Wild, S. M. Nazarewicz, W. TI Uncertainty Quantification for Nuclear Density Functional Theory and Information Content of New Measurements SO PHYSICAL REVIEW LETTERS LA English DT Article ID SENSITIVITY-ANALYSIS; BAYESIAN-INFERENCE; PHYSICS; SIMULATION; PROJECT; SYSTEMS AB Statistical tools of uncertainty quantification can be used to assess the information content of measured observables with respect to present-day theoretical models, to estimate model errors and thereby improve predictive capability, to extrapolate beyond the regions reached by experiment, and to provide meaningful input to applications and planned measurements. To showcase new opportunities offered by such tools, we make a rigorous analysis of theoretical statistical uncertainties in nuclear density functional theory using Bayesian inference methods. By considering the recent mass measurements from the Canadian Penning Trap at Argonne National Laboratory, we demonstrate how the Bayesian analysis and a direct least-squares optimization, combined with high-performance computing, can be used to assess the information content of the new data with respect to a model based on the Skyrme energy density functional approach. Employing the posterior probability distribution computed with a Gaussian process emulator, we apply the Bayesian framework to propagate theoretical statistical uncertainties in predictions of nuclear masses, two-neutron dripline, and fission barriers. Overall, we find that the new mass measurements do not impose a constraint that is strong enough to lead to significant changes in the model parameters. The example discussed in this study sets the stage for quantifying and maximizing the impact of new measurements with respect to current modeling and guiding future experimental efforts, thus enhancing the experiment-theory cycle in the scientific method. C1 [McDonnell, J. D.] Francis Marion Univ, Dept Phys & Astron, Florence, SC 29501 USA. [McDonnell, J. D.; Schunck, N.] Lawrence Livermore Natl Lab, Div Phys, Livermore, CA 94551 USA. [Higdon, D.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Sarich, J.; Wild, S. M.] Argonne Natl Lab, Div Math & Comp Sci, Argonne, IL 60439 USA. [Nazarewicz, W.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Nazarewicz, W.] Michigan State Univ, NSCL FRIB Lab, E Lansing, MI 48824 USA. [Nazarewicz, W.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Nazarewicz, W.] Univ Warsaw, Fac Phys, Inst Theoret Phys, PL-00681 Warsaw, Poland. RP McDonnell, JD (reprint author), Francis Marion Univ, Dept Phys & Astron, Florence, SC 29501 USA. RI Wild, Stefan/P-4907-2016; OI Wild, Stefan/0000-0002-6099-2772; Schunck, Nicolas/0000-0002-9203-6849 FU U.S. Department of Energy, Office of Science, Office of Nuclear Physics [DE-AC52-07NA27344, DE-AC02-06CH11357, DE-SC0008511]; NNSA's Stewardship Science Academic Alliances Program [DE-NA0001820]; Livermore Computing Resource Center at Lawrence Livermore National Laboratory; Laboratory Computing Resource Center at Argonne National Laboratory FX We are grateful to Guy Savard and Robert Janssens for helpful discussions and access to CPT masses. This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics under Awards No. DE-AC52-07NA27344 (Lawrence Livermore National Laboratory), No. DE-AC02-06CH11357 (Argonne National Laboratory), and No. DE-SC0008511 (NUCLEI SciDAC Collaboration), and by the NNSA's Stewardship Science Academic Alliances Program under Grant No. DE-NA0001820. Computational resources were provided through an INCITE award "Computational Nuclear Structure" by the National Center for Computational Sciences and National Institute for Computational Sciences at Oak Ridge National Laboratory, through a grant by the Livermore Computing Resource Center at Lawrence Livermore National Laboratory, and through a grant by the Laboratory Computing Resource Center at Argonne National Laboratory. NR 44 TC 14 Z9 14 U1 1 U2 17 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 24 PY 2015 VL 114 IS 12 AR 122501 DI 10.1103/PhysRevLett.114.122501 PG 6 WC Physics, Multidisciplinary SC Physics GA CH3GF UT WOS:000353916300003 PM 25860736 ER PT J AU Lee, E Kim, DH Denlinger, JD Kim, J Kim, K Min, BI Min, BH Kwon, YS Kang, JS AF Lee, Eunsook Kim, D. H. Denlinger, J. D. Kim, Junwon Kim, Kyoo Min, B. I. Min, B. H. Kwon, Y. S. Kang, J. -S. TI Angle-resolved and resonant photoemission spectroscopy study of the Fermi surface reconstruction in the charge density wave systems CeTe2 and PrTe2 SO PHYSICAL REVIEW B LA English DT Article ID ELECTRONIC-STRUCTURE; CRYSTAL-STRUCTURE; CE COMPOUNDS; SOLIDS; SPECTRA; MODEL; PR AB The electronic structures of a charge density wave (CDW) system RTe2 (R = Ce, Pr) have been investigated by employing angle-resolved photoemission spectroscopy (ARPES) and the first-principles band structure method. The R 4f hybridization peak (4f(n)c(m-1)) in the R 4f PES spectrum is located deeper in PrTe2 than in CeTe2 and R 4f spectral intensity near EF is much weaker in PrTe2 than in CeTe2, implying the importance of the hybridization between Ce 4f and Te(1) 5p electrons. For both CeTe2 and PrTe2, the metallic states crossing the Fermi level (EF) are observed below the CDW transition temperature, indicating the existence of the partially ungapped Fermi surfaces (FSs). The zigzag features having the fourfold rotational symmetry are observed near the X point in the FS of CeTe2, but not in the FS of PrTe2. The tight-binding model calculations show that the zigzag FS features in CeTe2 can be described as the CDW-induced FS reconstruction due to the 4 x 4 CDW supercell structure. The effect of the linear dichroism is observed in ARPES, suggesting that the E-F-crossing states have mainly the in-plane orbital character. The photon-energy maps for the near-E-F states exhibit the straight vertical dispersions for both CeTe2 and PrTe2, demonstrating the dominant two-dimensional character in RTe2 (R = Ce, Pr). C1 [Lee, Eunsook; Kim, D. H.; Kang, J. -S.] Catholic Univ Korea, Dept Phys, Bucheon 420743, South Korea. [Denlinger, J. D.] Lawrence Berkeley Natl Lab, ALS, Berkeley, CA USA. [Kim, Junwon; Kim, Kyoo; Min, B. I.] Pohang Univ Sci & Technol, POSTECH, Dept Phys, Pohang 790784, South Korea. [Min, B. H.; Kwon, Y. S.] DGIST, Dept Emerging Mat Sci, Daegu 711873, South Korea. RP Lee, E (reprint author), Catholic Univ Korea, Dept Phys, Bucheon 420743, South Korea. EM kangjs@catholic.ac.kr OI Kim, Kyoo/0000-0002-7305-8786 FU National Research Foundation (NRF) [2014R1A1A2056546, 2011-0025237]; POSTECH-BSRI grant; Korea Institute of Science and Technology Information (KISTI) supercomputing center [KSC-2013-C3-010]; US DOE [DE-AC0-205CH11231]; Basic Science Research Program of the NRF [2013R1A1A2009778]; Leading Foreign Research Institute Recruitment Program [2012K1A4A3053565]; Ministry of Science, ICT and Future Planning (MSIP) and Pohang Accelerator Laboratory (PAL) in Korea FX This work was supported by the National Research Foundation (NRF) under Contracts No. 2014R1A1A2056546 and No. 2011-0025237, the POSTECH-BSRI grant, and the Korea Institute of Science and Technology Information (KISTI) supercomputing center (No. KSC-2013-C3-010). The ALS is supported by US DOE under Contract No. DE-AC0-205CH11231. Y.S.K. and B.H.M. were supported by the Basic Science Research Program of the NRF (2013R1A1A2009778) and the Leading Foreign Research Institute Recruitment Program (Grant No. 2012K1A4A3053565). The travel for the ARPES experiment at the ALS was supported in part by the Ministry of Science, ICT and Future Planning (MSIP) and Pohang Accelerator Laboratory (PAL) in Korea. NR 35 TC 2 Z9 2 U1 2 U2 16 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAR 24 PY 2015 VL 91 IS 12 AR UNSP 125137 DI 10.1103/PhysRevB.91.125137 PG 7 WC Physics, Condensed Matter SC Physics GA CH3EQ UT WOS:000353910700003 ER PT J AU Abe, K Haga, Y Hayato, Y Ikeda, M Iyogi, K Kameda, J Kishimoto, Y Miura, M Moriyama, S Nakahata, M Nakano, Y Nakayama, S Sekiya, H Shiozawa, M Suzuki, Y Takeda, A Tanaka, H Tomura, T Ueno, K Wendell, RA Yokozawa, T Irvine, T Kajita, T Kametani, I Kaneyuki, K Lee, KP McLachlan, T Nishimura, Y Richard, E Okumura, K Labarga, L Fernandez, P Gustafson, J Kearns, E Raaf, JL Stone, JL Sulak, LR Berkman, S Tanaka, HA Tobayama, S Goldhaber, M Carminati, G Kropp, WR Mine, S Weatherly, P Renshaw, A Smy, MB Sobel, HW Takhistov, V Ganezer, KS Hartfiel, BL Hill, J Keig, WE Hong, N Kim, JY Lim, IT Akiri, T Himmel, A Scholberg, K Walter, CW Wongjirad, T Ishizuka, T Tasaka, S Jang, JS Learned, JG Matsuno, S Smith, SN Hasegawa, T Ishida, T Ishii, T Kobayashi, T Nakadaira, T Nakamura, K Oyama, Y Sakashita, K Sekiguchi, T Tsukamoto, T Suzuki, AT Takeuchi, Y Bronner, C Hirota, S Huang, K Ieki, K Kikawa, T Minamino, A Murakami, A Nakaya, T Suzuki, K Takahashi, S Tateishi, K Fukuda, Y Choi, K Itow, Y Mitsuka, G Mijakowski, P Hignight, J Imber, J Jung, CK Yanagisawa, C Ishino, H Kibayashi, A Koshio, Y Mori, T Sakuda, M Yamaguchi, R Yano, T Kuno, Y Tacik, R Kim, SB Okazawa, H Choi, Y Nishijima, K Koshiba, M Suda, Y Totsuka, Y Yokoyama, M Martens, K Marti, L Vagins, MR Martin, JF de Perio, P Konaka, A Wilking, MJ Chen, S Zhang, Y Connolly, K Wilkes, RJ AF Abe, K. Haga, Y. Hayato, Y. Ikeda, M. Iyogi, K. Kameda, J. Kishimoto, Y. Miura, M. Moriyama, S. Nakahata, M. Nakano, Y. Nakayama, S. Sekiya, H. Shiozawa, M. Suzuki, Y. Takeda, A. Tanaka, H. Tomura, T. Ueno, K. Wendell, R. A. Yokozawa, T. Irvine, T. Kajita, T. Kametani, I. Kaneyuki, K. Lee, K. P. McLachlan, T. Nishimura, Y. Richard, E. Okumura, K. Labarga, L. Fernandez, P. Gustafson, J. Kearns, E. Raaf, J. L. Stone, J. L. Sulak, L. R. Berkman, S. Tanaka, H. A. Tobayama, S. Goldhaber, M. Carminati, G. Kropp, W. R. Mine, S. Weatherly, P. Renshaw, A. Smy, M. B. Sobel, H. W. Takhistov, V. Ganezer, K. S. Hartfiel, B. L. Hill, J. Keig, W. E. Hong, N. Kim, J. Y. Lim, I. T. Akiri, T. Himmel, A. Scholberg, K. Walter, C. W. Wongjirad, T. Ishizuka, T. Tasaka, S. Jang, J. S. Learned, J. G. Matsuno, S. Smith, S. N. Hasegawa, T. Ishida, T. Ishii, T. Kobayashi, T. Nakadaira, T. Nakamura, K. Oyama, Y. Sakashita, K. Sekiguchi, T. Tsukamoto, T. Suzuki, A. T. Takeuchi, Y. Bronner, C. Hirota, S. Huang, K. Ieki, K. Kikawa, T. Minamino, A. Murakami, A. Nakaya, T. Suzuki, K. Takahashi, S. Tateishi, K. Fukuda, Y. Choi, K. Itow, Y. Mitsuka, G. Mijakowski, P. Hignight, J. Imber, J. Jung, C. K. Yanagisawa, C. Ishino, H. Kibayashi, A. Koshio, Y. Mori, T. Sakuda, M. Yamaguchi, R. Yano, T. Kuno, Y. Tacik, R. Kim, S. B. Okazawa, H. Choi, Y. Nishijima, K. Koshiba, M. Suda, Y. Totsuka, Y. Yokoyama, M. Martens, K. Marti, Ll. Vagins, M. R. Martin, J. F. de Perio, P. Konaka, A. Wilking, M. J. Chen, S. Zhang, Y. Connolly, K. Wilkes, R. J. CA Super Kamiokande Collaboration TI Limits on sterile neutrino mixing using atmospheric neutrinos in Super-Kamiokande SO PHYSICAL REVIEW D LA English DT Article ID OSCILLATIONS; DETECTOR; GALLEX; RANGE; MODEL AB We present limits on sterile neutrino mixing using 4,438 live-days of atmospheric neutrino data from the Super-Kamiokande experiment. We search for fast oscillations driven by an eV(2)-scale mass splitting and for oscillations into sterile neutrinos instead of tau neutrinos at the atmospheric mass splitting. When performing both of these searches we assume that the sterile mass splitting is large, allowing sin(2) (Delta m(2)L/4E) to be approximated as 0.5, and we assume that there is no mixing between electron neutrinos and sterile neutrinos (vertical bar U-e4 vertical bar(2) = 0). No evidence of sterile oscillations is seen and we limit vertical bar U-mu 4 vertical bar(2) to less than 0.041 and vertical bar U-tau 4 vertical bar(2) to less than 0.18 for Delta m(2) > 0.1 eV(2) at the 90% C.L. in a 3 + 1 framework. The approximations that can be made with atmospheric neutrinos allow these limits to be easily applied to 3 + N models, and we provide our results in a generic format to allow comparisons with other sterile neutrino models. C1 [Abe, K.; Haga, Y.; Hayato, Y.; Ikeda, M.; Iyogi, K.; Kameda, J.; Kishimoto, Y.; Miura, M.; Moriyama, S.; Nakahata, M.; Nakano, Y.; Nakayama, S.; Sekiya, H.; Shiozawa, M.; Suzuki, Y.; Takeda, A.; Tanaka, H.; Tomura, T.; Ueno, K.; Wendell, R. A.; Yokozawa, T.; Himmel, A.] Univ Tokyo, Inst Cosm Ray Res, Kamioka Observ, Kamioka, Gifu 5061205, Japan. [Irvine, T.; Kajita, T.; Kametani, I.; Kaneyuki, K.; Lee, K. P.; McLachlan, T.; Richard, E.; Okumura, K.] Univ Tokyo, Inst Cosm Ray Res, Res Ctr Cosm Neutrinos, Kashiwa, Chiba 2778582, Japan. [Labarga, L.; Fernandez, P.] Univ Autonoma Madrid, Dept Phys Theor, E-28049 Madrid, Spain. [Berkman, S.; Tanaka, H. A.; Tobayama, S.] Univ British Columbia, Dept Phys & Astron, Vancouver, BC V6T 1Z4, Canada. [Goldhaber, M.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Carminati, G.; Kropp, W. R.; Mine, S.; Weatherly, P.; Renshaw, A.; Smy, M. B.; Sobel, H. W.; Takhistov, V.; Vagins, M. R.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. [Ganezer, K. S.; Hartfiel, B. L.; Hill, J.; Keig, W. E.] Calif State Univ Dominguez Hills, Dept Phys, Carson, CA 90747 USA. [Hong, N.; Kim, J. Y.; Lim, I. T.] Chonnam Natl Univ, Dept Phys, Kwangju 500757, South Korea. [Akiri, T.; Himmel, A.; Scholberg, K.; Walter, C. W.; Wongjirad, T.] Duke Univ, Dept Phys, Durham, NC 27708 USA. [Ishizuka, T.] Fukuoka Inst Technol, Junior Coll, Fukuoka, Fukuoka 8110295, Japan. [Tasaka, S.] Gifu Univ, Dept Phys, Gifu, Gifu 5011193, Japan. [Jang, J. S.] Gwangju Inst Sci & Technol, GIST Coll, Kwangju 500712, South Korea. [Learned, J. G.; Matsuno, S.; Smith, S. N.] Univ Hawaii, Dept Phys & Astron, Honolulu, HI 96822 USA. [Hasegawa, T.; Ishida, T.; Ishii, T.; Kobayashi, T.; Nakadaira, T.; Nakamura, K.; Oyama, Y.; Sakashita, K.; Sekiguchi, T.; Tsukamoto, T.] High Energy Accelerator Res Org KEK, Tsukuba, Ibaraki 3050801, Japan. [Suzuki, A. T.; Takeuchi, Y.] Kobe Univ, Dept Phys, Kobe, Hyogo 6578501, Japan. [Bronner, C.; Hirota, S.; Huang, K.; Ieki, K.; Kikawa, T.; Minamino, A.; Murakami, A.; Nakaya, T.; Suzuki, K.; Takahashi, S.; Tateishi, K.] Kyoto Univ, Dept Phys, Kyoto, Kyoto 6068502, Japan. [Fukuda, Y.] Miyagi Univ Educ, Dept Phys, Sendai, Miyagi 9800845, Japan. [Choi, K.; Itow, Y.; Mitsuka, G.] Nagoya Univ, Solar Terr Environm Lab, Nagoya, Aichi 4648602, Japan. [Hignight, J.; Imber, J.; Jung, C. K.; Yanagisawa, C.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Ishino, H.; Kibayashi, A.; Koshio, Y.; Mori, T.; Sakuda, M.; Yamaguchi, R.; Yano, T.] Okayama Univ, Dept Phys, Okayama, Okayama 7008530, Japan. [Tacik, R.] Univ Regina, Dept Phys, Regina, SK S4S OA2, Canada. [Kim, S. B.] Seoul Natl Univ, Dept Phys, Seoul 151742, South Korea. [Okazawa, H.] Shizuoka Univ Welf, Dept Informat Social Welf, Shizuoka 4258611, Japan. [Choi, Y.] Sungkyunkwan Univ, Dept Phys, Suwon 440746, South Korea. [Nishijima, K.] Tokai Univ, Dept Phys, Hiratsuka, Kanagawa 2591292, Japan. [Koshiba, M.; Suda, Y.; Totsuka, Y.; Yokoyama, M.] Univ Tokyo, Bunkyo Ku, Tokyo 1130033, Japan. [Abe, K.; Hayato, Y.; Kameda, J.; Kishimoto, Y.; Miura, M.; Moriyama, S.; Nakahata, M.; Nakayama, S.; Sekiya, H.; Shiozawa, M.; Suzuki, Y.; Takeda, A.; Tomura, T.; Wendell, R. A.; Kametani, I.; Okumura, K.; Kearns, E.; Stone, J. L.; Smy, M. B.; Sobel, H. W.; Scholberg, K.; Walter, C. W.; Nakamura, K.; Nakaya, T.; Yokoyama, M.; Martens, K.; Marti, Ll.; Vagins, M. R.] Univ Tokyo, Todai Inst Adv Study, Kavli Inst Phys & Math Univ WPI, Kashiwa, Chiba 2778582, Japan. [Martin, J. F.; de Perio, P.] Univ Toronto, Dept Phys, Toronto, ON M5S 1A7, Canada. [Tacik, R.; Konaka, A.; Wilking, M. J.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Nishimura, Y.; Chen, S.; Zhang, Y.] Tsinghua Univ, Dept Engn Phys, Beijing 100084, Peoples R China. [Connolly, K.; Wilkes, R. J.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Mijakowski, P.] Natl Ctr Nucl Res, PL-00681 Warsaw, Poland. RP Abe, K (reprint author), Univ Tokyo, Inst Cosm Ray Res, Kamioka Observ, Kamioka, Gifu 5061205, Japan. RI Ishino, Hirokazu/C-1994-2015; Kibayashi, Atsuko/K-7327-2015; Koshio, Yusuke/C-2847-2015; Nakano, Yuuki/S-2684-2016; Yokoyama, Masashi/A-4458-2011 OI Ishino, Hirokazu/0000-0002-8623-4080; Koshio, Yusuke/0000-0003-0437-8505; Yokoyama, Masashi/0000-0003-2742-0251 FU Japanese Ministry of Education, Culture, Sports, Science and Technology; U.S. Department of Energy; U.S. National Science Foundation; Research Foundation of Korea (BK21); Research Foundation of Korea (KNRC); Korean Ministry of Science and Technology; National Science Foundation of China; European Union [PN-284518, GA-2011-289442]; National Science and Engineering Research Council (NSERC) of Canada; Scinet and Westgrid consortia of Compute Canada FX The authors would like to thank M. Maltoni for his help calculating and implementing the sterile oscillation probabilities. The authors gratefully acknowledge the cooperation of the Kamioka Mining and Smelting Company. Super-K has been built and operated from funds provided by the Japanese Ministry of Education, Culture, Sports, Science and Technology, the U.S. Department of Energy, and the U.S. National Science Foundation. This work was partially supported by the Research Foundation of Korea (BK21 and KNRC), the Korean Ministry of Science and Technology, the National Science Foundation of China, the European Union FP7 (DS laguna-lbno PN-284518 and ITN invisibles GA-2011-289442) the National Science and Engineering Research Council (NSERC) of Canada, and the Scinet and Westgrid consortia of Compute Canada. NR 70 TC 15 Z9 15 U1 0 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 24 PY 2015 VL 91 IS 5 AR 052019 DI 10.1103/PhysRevD.91.052019 PG 22 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CH3FM UT WOS:000353913800001 ER PT J AU Sava Gallis, DF Parkes, MV Greathouse, JA Zhang, XY Nenoff, TM AF Sava Gallis, Dorina F. Parkes, Marie V. Greathouse, Jeffery A. Zhang, Xiaoyi Nenoff, Tina M. TI Enhanced O-2 Selectivity versus N-2 by Partial Metal Substitution in Cu-BTC SO CHEMISTRY OF MATERIALS LA English DT Article ID AUGMENTED-WAVE METHOD; ORGANIC FRAMEWORKS; GAS-ADSORPTION; CO2 ADSORPTION; HYDROGEN ADSORPTION; CARBON CAPTURE; STORAGE; BINDING; OXYGEN; SITES AB Here, we describe the homogeneous substitution of Mn, Fe, and Co at various levels into a prototypical metal organic framework (MOP), namely Cu-BTC (HKUST-1), and the effect of that substitution on preferential gas sorption. Using a combination of density functional theory (DFT) calculations, postsynthetic metal substitutions, materials characterization, and gas sorption testing, we demonstrate that the identity of the metal ion has a quantifiable effect on their oxygen and nitrogen sorption properties at cryogenic temperatures. An excellent correlation is found between O-2/N-2 selectivities determined experimentally at 77 K and the difference in O-2 and N-2 binding energies calculated from DFT modeling data: Mn > Fe Co >> Cu. Room temperature gas sorption studies were also performed and correlated with metal substitution. The Fe-exchanged sample shows a significantly higher nitrogen isosteric heat of adsorption at temperatures close to ambient conditions (273-298 K) as compared to all other metals studied, indicative of favorable interactions between N-2 and coordinatively unsaturated Fe metal centers. Interestingly, differences in gas adsorption results at cryogenic and room temperatures are evident; they are explained by comparing experimental results with DFT binding energies (0 K) and room temperature Grand Canonical Monte Carlo simulations. C1 [Sava Gallis, Dorina F.; Nenoff, Tina M.] Sandia Natl Labs, Nanoscale Sci Dept, Albuquerque, NM 87185 USA. [Parkes, Marie V.; Greathouse, Jeffery A.] Sandia Natl Labs, Geochem Dept, Albuquerque, NM 87185 USA. [Zhang, Xiaoyi] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. RP Nenoff, TM (reprint author), Sandia Natl Labs, Nanoscale Sci Dept, POB 5800, Albuquerque, NM 87185 USA. EM tmnenof@sandia.gov RI Sava Gallis, Dorina/D-2827-2015 FU U.S. DOE's NNSA [DE-AC04-94AL85000]; U.S. DOE [DE-AC02-06CH11357] FX The authors would like to acknowledge Mark A. Rodriguez for his help with PXRD unit cell refinement and helpful discussions. This work is supported by the Laboratory Directed Research and Development Program at Sandia National Laboratories. Sandia National Laboratories is a multiprogram lab managed and operated by Sandia Corp., a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. DOE's NNSA under contract DE-AC04-94AL85000. Work done at Argonne and use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. DOE/Office of Science by Argonne National Laboratory, was supported by the U.S. DOE, Contract No. DE-AC02-06CH11357. NR 59 TC 10 Z9 10 U1 12 U2 83 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD MAR 24 PY 2015 VL 27 IS 6 BP 2018 EP 2025 DI 10.1021/cm5042293 PG 8 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CE6TR UT WOS:000351971600016 ER PT J AU Quinn, NWT Burns, JR AF Quinn, Nigel W. T. Burns, Jos R. TI Use of a hybrid optical remote sensing classification technique for seasonal wetland habitat degradation assessment resulting from adoption of real-time salinity management practices SO JOURNAL OF APPLIED REMOTE SENSING LA English DT Article DE wetland vegetation; salt management; remote sensing; waterfowl habitat; total maximum daily load ID SPECTRAL DISCRIMINATION; COASTAL WETLANDS; VEGETATION TYPES; CALIFORNIA; IMAGERY; PHOTOGRAPHY; SYSTEM; GIS AB Delayed seasonal wetland drawdown is being investigated as one means of improving the scheduling of saline drainage discharge to the San Joaquin River, California, as an application of the principal of basin-scale real-time salinity management. A hybrid rapid vegetation assessment methodology was derived from the California Native Plant Society Rapid Assessment Protocol for classifying the vegetation in these seasonal wetlands. A hybrid remote sensing methodology combining pixel- and object-based components was developed to apply this classification strategy to a 160 km(2) region. Twenty-six different plant communities were represented in a total of 20 land cover classes. An overall mapping accuracy ranges from 60% for identification of all 26 plant communities to 100% for identification of a single plant species. Low representation of certain associations for sensor calibration resulted in lower than anticipated mapping success as measured by errors of omission and commission. This image processing methodology provides an important tool, in concert with soil salinity mapping and wetland biology surveys, to assess the long-term impact of adaptive management strategies such as real-time salinity management on the wetland resource. (C) The Authors. Published by SPIE under a Creative Commons Attribution 3.0 Unported License. C1 [Quinn, Nigel W. T.; Burns, Jos R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, HydroEcol Engn Adv Decis Support, Berkeley, CA 94720 USA. RP Quinn, NWT (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, HydroEcol Engn Adv Decis Support, 1 Cyclotron Rd,MS 64-209, Berkeley, CA 94720 USA. EM nwquinn@lbl.gov RI Quinn, Nigel/G-2407-2015 OI Quinn, Nigel/0000-0003-3333-4763 FU State Water Resources Control Board; US Bureau of Reclamation; California Department of Water Resources; U.S. Department of Energy; LBNL [DE-AC02-05CH11231] FX The authors are indebted to the State Water Resources Control Board, US Bureau of Reclamation and California Department of Water Resources for grant funding in support of this ongoing research. Thanks also to the Grassland Water District, Salinas Land and Cattle Club, California Department of Fish and Game, and U.S. Fish and Wildlife Service on whose lands the study was been carried out. Of particular note is Jeff Milliken (US Bureau of Reclamation), who provided technical assistance on ERDAS Imagine and Definiens eCognition modeling, Tim Poole (Salinas Land and Cattle Club) for his help in vegetation identification, and Ricardo Ortega and Lara Sparks (California Department of Fish and Game), who assisted with various aspects of field data acquisition, vegetation surveys, and ground truthing. This research was also supported by the U.S. Department of Energy and LBNL under Contract No. DE-AC02-05CH11231. NR 54 TC 0 Z9 0 U1 9 U2 23 PU SPIE-SOC PHOTO-OPTICAL INSTRUMENTATION ENGINEERS PI BELLINGHAM PA 1000 20TH ST, PO BOX 10, BELLINGHAM, WA 98225 USA SN 1931-3195 J9 J APPL REMOTE SENS JI J. Appl. Remote Sens. PD MAR 24 PY 2015 VL 9 AR 096071 DI 10.1117/1.JRS.9.096071 PG 25 WC Environmental Sciences; Remote Sensing; Imaging Science & Photographic Technology SC Environmental Sciences & Ecology; Remote Sensing; Imaging Science & Photographic Technology GA CF8TO UT WOS:000352835000001 ER PT J AU Park, JS Mane, AU Elam, JW Croy, JR AF Park, Joong Sun Mane, Anil U. Elam, Jeffrey W. Croy, Jason R. TI Amorphous Metal Fluoride Passivation Coatings Prepared by Atomic Layer Deposition on LiCoO2 for Li-Ion Batteries SO CHEMISTRY OF MATERIALS LA English DT Article ID RECHARGEABLE LITHIUM BATTERIES; VOLTAGE CYCLING BEHAVIOR; CATHODE MATERIALS; THIN-FILMS; PARTICLES; ELECTRODES; STABILITY; ALUMINA; AL2O3; TIF4 C1 [Park, Joong Sun; Croy, Jason R.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Mane, Anil U.; Elam, Jeffrey W.] Argonne Natl Lab, Div Energy Syst, Argonne, IL 60439 USA. RP Croy, JR (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM croy@anl.gov FU Batteries for Advanced Transportation Technologies (BATT) Program; Center for Electrochemical Energy Science, an Energy Frontier Research Center - U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES) FX Support from the Batteries for Advanced Transportation Technologies (BATT) Program, in particular David Howell and Tien Duong, of the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, is gratefully acknowledged. This research was supported as part of the Center for Electrochemical Energy Science, an Energy Frontier Research Center funded by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES) (ALD coatings and characterization). NR 39 TC 13 Z9 13 U1 9 U2 98 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD MAR 24 PY 2015 VL 27 IS 6 BP 1917 EP 1920 DI 10.1021/acs.chemmater.5b00603 PG 4 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CE6TR UT WOS:000351971600003 ER PT J AU Dayal, S Zhong, HZ Kopidakis, N Scholes, GD Rumbles, G AF Dayal, Smita Zhong, Haizheng Kopidakis, Nikos Scholes, Gregory D. Rumbles, Garry TI Improved power conversion efficiency for bulk heterojunction solar cells incorporating CdTe-CdSe nanoheterostructure acceptors and a conjugated polymer donor SO JOURNAL OF PHOTONICS FOR ENERGY LA English DT Article DE nanoheterostructures; photovoltaic devices; solar power conversion efficiency; p3HT; PCPDTBT ID COLLOIDAL NANOCRYSTAL HETEROSTRUCTURES; PHOTOVOLTAIC CELLS; SEMICONDUCTOR NANOCRYSTALS; CHARGE SEPARATION; NANORODS; PERFORMANCE; SHAPE; POLY(3-HEXYLTHIOPHENE); NANOPARTICLES; DYNAMICS AB We report photovoltaic devices based on composites of a branched nanoheterostructure containing a CdTe core and CdSe arms, CdTe(c)-CdSe(a), combined with either poly(3-hexylthiophene), P3HT, or poly[2,6-(4,4-bis-(2-ethylhexyl)-4H-cyclopenta[2,1-b;3,4-b']dithiophene)-alt-4,7-(2,1,3-benzothiadiazole)], PCPDTBT, with solar power conversion efficiencies of 1.2% and 1.8%, respectively. A comparison with previously reported composite devices of a related branched nanoheterostructure: CdSe(c)-CdTe(a) reveals an improved device performance that is attributed to a better electron percolation pathway provided by the dominant, higher electron affinity CdSe arms of the nanoheterostructures. (C) 2015 Society of Photo-Optical Instrumentation Engineers (SPIE) C1 [Dayal, Smita; Kopidakis, Nikos; Rumbles, Garry] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Zhong, Haizheng] Beijing Inst Technol, Sch Mat Sci & Engn, Micro Nano Res Ctr, Beijing 100081, Peoples R China. [Scholes, Gregory D.] Princeton Univ, Dept Chem, Princeton, NJ 08544 USA. RP Rumbles, G (reprint author), Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. EM Garry.Rumbles@nrel.gov RI Kopidakis, Nikos/N-4777-2015 FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences [DE-AC36- 08GO28308]; Natural Sciences and Engineering Research Council of Canada (NSERC) FX The electron transfer studies were funded by the solar photochemistry program of the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences, under Contract No. DE-AC36- 08GO28308 to National Renewable Energy Laboratory (NREL). Synthesis and characterization of the nanoheterostructures were funded by the Natural Sciences and Engineering Research Council of Canada (NSERC). NR 40 TC 3 Z9 3 U1 5 U2 27 PU SPIE-SOC PHOTO-OPTICAL INSTRUMENTATION ENGINEERS PI BELLINGHAM PA 1000 20TH ST, PO BOX 10, BELLINGHAM, WA 98225 USA SN 1947-7988 J9 J PHOTON ENERGY JI J. Photonics Energy PD MAR 24 PY 2015 VL 5 AR 057409 DI 10.1117/1.JPE.5.057409 PG 9 WC Materials Science, Multidisciplinary; Optics; Physics, Applied SC Materials Science; Optics; Physics GA CF8YA UT WOS:000352846800001 ER PT J AU Giera, B Henson, N Kober, EM Shell, MS Squires, TM AF Giera, Brian Henson, Neil Kober, Edward M. Shell, M. Scott Squires, Todd M. TI Electric Double-Layer Structure in Primitive Model Electrolytes: Comparing Molecular Dynamics with Local-Density Approximations SO LANGMUIR LA English DT Article ID EQUATION-OF-STATE; PERTURBATION-THEORY; IONIC LIQUIDS; FLUIDS; INTERFACE; SPHERES AB We evaluate the accuracy of local-density approximations (LDAs) using explicit molecular dynamics simulations of binary electrolytes comprised of equisized ions in an implicit solvent. The Bikerman LDA, which considers ions to occupy a lattice, poorly captures excluded volume interactions between primitive model ions. Instead, LDAs based on the Carnahan-Starling (CS) hard-sphere equation of state capture simulated values of ideal and excess chemical potential profiles extremely well, as well as the relationship between surface charge density and electrostatic potential. Excellent agreement between the EDL capacitances predicted by CS-LDAs and computed in molecular simulations is found even in systems where ion correlations drive strong density and free charge oscillations within the EDL, despite the inability of LDAs to capture the oscillations in the detailed EDL profiles. C1 [Giera, Brian; Shell, M. Scott; Squires, Todd M.] Univ Calif Santa Barbara, Dept Chem Engn, Santa Barbara, CA 93106 USA. [Giera, Brian] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Henson, Neil; Kober, Edward M.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Squires, TM (reprint author), Univ Calif Santa Barbara, Dept Chem Engn, Santa Barbara, CA 93106 USA. EM squires@engineering.ucsb.edu OI Henson, Neil/0000-0002-1842-7884 FU U.S. Department of Energy through Los Alamos National Laboratory/UCSB Institute for Multiscale Materials Studies; W. M. Keck Foundation; UCSB Doctoral Scholars Graduate Fellowship; Lawrence Livemore National Laboratory [DE-AC52-07NA27344] FX We gratefully acknowledge primary support from the U.S. Department of Energy through the Los Alamos National Laboratory/UCSB Institute for Multiscale Materials Studies and partial support from the W. M. Keck Foundation, the UCSB Doctoral Scholars Graduate Fellowship, and Lawrence Livemore National Laboratory under contract DE-AC52-07NA27344. NR 44 TC 10 Z9 10 U1 7 U2 42 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0743-7463 J9 LANGMUIR JI Langmuir PD MAR 24 PY 2015 VL 31 IS 11 BP 3553 EP 3562 DI 10.1021/la5048936 PG 10 WC Chemistry, Multidisciplinary; Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CE4HX UT WOS:000351792800032 PM 25723189 ER PT J AU Wolfsgruber, S Jessen, F Koppara, A Kleineidam, L Schmidtke, K Frolich, L Kurz, A Schulz, S Hampel, H Heuser, I Peters, O Reischies, FM Jahn, H Luckhaus, C Hull, M Gertz, HJ Schroder, J Pantel, J Rienhoff, O Ruther, E Henn, F Wiltfang, J Maier, W Kornhuber, J Wagner, M AF Wolfsgruber, Steffen Jessen, Frank Koppara, Alexander Kleineidam, Luca Schmidtke, Klaus Froelich, Lutz Kurz, Alexander Schulz, Stefanie Hampel, Harald Heuser, Isabella Peters, Oliver Reischies, Friedel M. Jahn, Holger Luckhaus, Christian Huell, Michael Gertz, Hermann-Josef Schroeder, Johannes Pantel, Johannes Rienhoff, Otto Ruether, Eckart Henn, Fritz Wiltfang, Jens Maier, Wolfgang Kornhuber, Johannes Wagner, Michael TI Subjective cognitive decline is related to CSF biomarkers of AD in patients with MCI SO NEUROLOGY LA English DT Article ID ALZHEIMERS ASSOCIATION WORKGROUPS; MEMORY COMPLAINTS; DIAGNOSTIC GUIDELINES; NATIONAL INSTITUTE; AMYLOID BURDEN; AMNESTIC MCI; OLDER-ADULTS; CUED-RECALL; DISEASE; IMPAIRMENT AB Objective: To test whether, in individuals with mild cognitive impairment (MCI), different measures of subjective cognitive decline (SCD) in the memory domain predict abnormal CSF biomarkers of Alzheimer disease (AD). Methods: We analyzed the multicenter baseline (cross-sectional) data of 245 patients with MCI. SCD was measured quantitatively with the Subjective Memory Decline Scale (SMDS) and qualitatively by assessing particular concerns associated with self-experienced worsening of memory. Logistic regression models were used to examine associations between SCD and abnormal CSF biomarkers, taking into account objective memory impairment, depressive symptoms, and education as covariates. Results: Abnormal CSF beta-amyloid 1-42 (A beta 42) and more depressive symptoms were associated with higher SMDS scores and with the report of memory concerns. Risk of abnormal CSF A beta 42 increased by an estimated 57% for a 1-SD increase in SMDS scores and was doubled in patients who had SMDS scores >4 or who reported memory concerns, respectively. In addition, both SCD measures predicted risk of having a biomarker signature indicative of prodromal AD defined as presence of low CSF A beta 42 together with either high CSF tau or CSF phosphorylated tau 181 levels. Conclusions: In MCI, specific aspects of SCD severity and quality are related to CSF biomarkers indicative of AD. This extends findings in pre-MCI samples and calls for an improved operational assessment of SCD in MCI. This might be useful for sample enrichment strategies for increased likelihood of AD pathology. C1 [Wolfsgruber, Steffen; Jessen, Frank; Koppara, Alexander; Kleineidam, Luca; Maier, Wolfgang; Wagner, Michael] Univ Bonn, Dept Psychiat, Bonn, Germany. [Wolfsgruber, Steffen; Jessen, Frank; Koppara, Alexander; Kleineidam, Luca; Maier, Wolfgang; Wagner, Michael] German Ctr Neurodegenerat Dis, Bonn, Germany. [Schmidtke, Klaus] Ortenau Klinikum, Ctr Geriatr Med, Offenburg Gengenbach, Germany. [Froelich, Lutz] Cent Inst Mental Hlth, Dept Gerontopsychiat, Mannheim, Germany. [Kurz, Alexander] Tech Univ Munich, Dept Psychiat, D-80290 Munich, Germany. [Schulz, Stefanie] Univ Aachen, Dept Neurol, Aachen, Germany. [Schulz, Stefanie; Ruether, Eckart; Wiltfang, Jens] Univ Gottingen, Dept Psychiat & Psychotherapy, Gottingen, Germany. [Hampel, Harald] Univ Paris 06, AXA Res Fund, Paris, France. [Hampel, Harald] Univ Paris 06, UPMC Chair Sorbonne Univ, Paris, France. [Hampel, Harald] Hop La Pitie Salpetriere, Inst Memoire & Maladie Alzheimer, Dept Neurol, Paris, France. [Hampel, Harald] INSERM, Inst Cerveau & Moelle Epiniere, U1127, Paris, France. [Heuser, Isabella; Peters, Oliver; Reischies, Friedel M.] Charite, Campus Benjamin Franklin, Dept Psychiat, Berlin, Germany. [Jahn, Holger] Univ Hamburg, Dept Psychiat, Hamburg, Germany. [Luckhaus, Christian] Univ Dusseldorf, Dept Psychiat, Dusseldorf, Germany. [Huell, Michael] Univ Freiburg, Ctr Geriatr Med & Gerontol, Freiburg, Germany. [Gertz, Hermann-Josef] Univ Leipzig, Dept Psychiat, D-04109 Leipzig, Germany. [Schroeder, Johannes] Heidelberg Univ, Dept Psychiat, D-69115 Heidelberg, Germany. [Pantel, Johannes] Goethe Univ Frankfurt, Dept Gen Med, D-60054 Frankfurt, Germany. [Rienhoff, Otto] Univ Gottingen, Dept Med Informat, Gottingen, Germany. [Henn, Fritz] Brookhaven Natl Lab, Upton, NY 11973 USA. [Kornhuber, Johannes] Univ Erlangen Nurnberg, Dept Psychiat, Nurnberg, Germany. RP Wolfsgruber, S (reprint author), Univ Bonn, Dept Psychiat, Bonn, Germany. EM steffen.wolfsgruber@ukb.uni-bonn.de RI Jahn, Holger/A-9255-2008; Wagner, Michael/E-2325-2011; Fachbereich14, Dekanat/C-8553-2015; OI Jahn, Holger/0000-0003-3607-7651; Wagner, Michael/0000-0003-2589-6440; Koppara, Alexander/0000-0002-3577-6349; Kornhuber, Johannes/0000-0002-8096-3987 FU German Federal Ministry of Education and Research (BMBF) [01GI0420]; Katharina-Hardt Foundation, Bad Homburg, Germany; AXA Research Fund; Fondation Universite Pierre et Marie Curie; Fondation pour la Recherche sur Alzheimer, Paris, France; program "Investissements d'avenir" [ANR-10-IAIHU-06] FX This study has been supported by a grant from the German Federal Ministry of Education and Research (BMBF): Kompetenznetz Demenzen (01GI0420). Harald Hampel was supported by grants of the Katharina-Hardt Foundation, Bad Homburg, Germany. He is further supported by the AXA Research Fund, the Fondation Universite Pierre et Marie Curie, and the Fondation pour la Recherche sur Alzheimer, Paris, France. The research leading to these results has received funding from the program "Investissements d'avenir" ANR-10-IAIHU-06. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 40 TC 9 Z9 9 U1 4 U2 17 PU LIPPINCOTT WILLIAMS & WILKINS PI PHILADELPHIA PA TWO COMMERCE SQ, 2001 MARKET ST, PHILADELPHIA, PA 19103 USA SN 0028-3878 EI 1526-632X J9 NEUROLOGY JI Neurology PD MAR 24 PY 2015 VL 84 IS 12 BP 1261 EP 1268 DI 10.1212/WNL.0000000000001399 PG 8 WC Clinical Neurology SC Neurosciences & Neurology GA CE2RI UT WOS:000351663200018 PM 25716354 ER PT J AU Sun, Y Gleber, SC Jacobsen, C Kirz, J Vogt, S AF Sun, Yue Gleber, Sophie-Charlotte Jacobsen, Chris Kirz, Janos Vogt, Stefan TI Optimizing detector geometry for trace element mapping by X-ray fluorescence SO ULTRAMICROSCOPY LA English DT Article DE Trace element detection; X-ray fluorescence; X-ray fluorescence microscopy; Detector geometry; Signal-to-noise ratio ID MONTE-CARLO-SIMULATION; HOMOGENEOUS SAMPLES; SYNCHROTRON-RADIATION; BIOLOGICAL-MATERIALS; FREE-ELECTRONS; SOLAR-CELLS; SCATTERING; SPECTROMETERS; MICROSCOPY; PIXE AB Trace metals play critical roles in a variety of systems, ranging from cells to photovoltaics. X-Ray Fluorescence (XRF) microscopy using X-ray excitation provides one of the highest sensitivities available for imaging the distribution of trace metals at sub-100 nm resolution. With the growing availability and increasing performance of synchrotron light source based instruments and X-ray nanofocusing optics, and with improvements in energy-dispersive XRF detectors, what are the factors that limit trace element detectability? To address this question, we describe an analytical model for the total signal incident on XRF detectors with various geometries, including the spectral response of energy dispersive detectors. This model agrees well with experimentally recorded X-ray fluorescence spectra, and involves much shorter calculation times than with Monte Carlo simulations. With such a model, one can estimate the signal when a trace element is illuminated with an X-ray beam, and when just the surrounding non fluorescent material is illuminated. From this signal difference, a contrast parameter can be calculated and this can in turn be used to calculate the signal-to-noise ratio (S/N) for detecting a certain elemental concentration. We apply this model to the detection of trace amounts of zinc in biological materials, and to the detection of small quantities of arsenic in semiconductors. We conclude that increased detector collection solid angle is (nearly) always advantageous even when considering the scattered signal. However, given the choice between a smaller detector at 90 degrees to the beam versus a larger detector at 180 degrees (in a backscatter-like geometry), the 90 degrees detector is better for trace element detection in thick samples, while the larger detector in 180 degrees geometry is better suited to trace element detection in thin samples. (C) 2015 Published by Elsevier B.V. C1 [Sun, Yue] Northwestern Univ, Grad Program Appl Phys, Evanston, IL 60208 USA. [Gleber, Sophie-Charlotte; Jacobsen, Chris; Vogt, Stefan] Argonne Natl Lab, Argonne, IL 60439 USA. [Kirz, Janos] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Jacobsen, Chris] Northwestern Univ, Dept Phys & Astron, Evanston, IL 60208 USA. [Jacobsen, Chris] Northwestern Univ, Chem Life Proc Inst, Evanston, IL 60208 USA. RP Vogt, S (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. EM ysun@u.northwestern.edu; gleber@aps.anl.gov; cjacobsen@anl.gov; jkirz@lbl.gov; vogt@aps.anl.gov RI Vogt, Stefan/B-9547-2009; Vogt, Stefan/J-7937-2013; Jacobsen, Chris/E-2827-2015 OI Vogt, Stefan/0000-0002-8034-5513; Vogt, Stefan/0000-0002-8034-5513; Jacobsen, Chris/0000-0001-8562-0353 FU US Department of Energy, Office of Science, Basic Energy Sciences program [DE-AC02-06CH11357]; National Institutes of Health [RO1 GM 104530] FX This work was supported by the US Department of Energy, Office of Science, Basic Energy Sciences program under contract DE-AC02-06CH11357, and by the National Institutes of Health under grant RO1 GM 104530, We would also like to thank Barry Lai for his support in the measurement at beamline 2IDD of the Advanced Photon Source, and Mark Rivers for his constructive suggestions. NR 58 TC 5 Z9 5 U1 2 U2 24 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0304-3991 EI 1879-2723 J9 ULTRAMICROSCOPY JI Ultramicroscopy PD MAR 24 PY 2015 VL 152 BP 44 EP 56 DI 10.1016/j.ultramic.2014.12.014 PG 13 WC Microscopy SC Microscopy GA CE6KK UT WOS:000351945100005 PM 25600825 ER PT J AU Siegel, JB Smith, AL Poust, S Wargacki, AJ Bar-Even, A Louw, C Shen, BW Eiben, CB Tran, HM Noor, E Gallaher, JL Bale, J Yoshikuni, Y Gelb, MH Keasling, JD Stoddard, BL Lidstrom, ME Baker, D AF Siegel, Justin B. Smith, Amanda Lee Poust, Sean Wargacki, Adam J. Bar-Even, Arren Louw, Catherine Shen, Betty W. Eiben, Christopher B. Tran, Huu M. Noor, Elad Gallaher, Jasmine L. Bale, Jacob Yoshikuni, Yasuo Gelb, Michael H. Keasling, Jay D. Stoddard, Barry L. Lidstrom, Mary E. Baker, David TI Computational protein design enables a novel one-carbon assimilation pathway SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE computational protein design; pathway engineering; carbon fixation ID ACETYL-COENZYME-A; ESCHERICHIA-COLI; PSEUDOMONAS-FLUORESCENS; FORMATE TRANSPORTER; BENZALDEHYDE LYASE; ENZYME; DEHYDROGENASE; METABOLITE; CONVERSION; MECHANISM AB We describe a computationally designed enzyme, formolase (FLS), which catalyzes the carboligation of three one-carbon formaldehyde molecules into one three-carbon dihydroxyacetone molecule. The existence of FLS enables the design of a new carbon fixation pathway, the formolase pathway, consisting of a small number of thermodynamically favorable chemical transformations that convert formate into a three-carbon sugar in central metabolism. The formolase pathway is predicted to use carbon more efficiently and with less backward flux than any naturally occurring one-carbon assimilation pathway. When supplemented with enzymes carrying out the other steps in the pathway, FLS converts formate into dihydroxyacetone phosphate and other central metabolites in vitro. These results demonstrate how modern protein engineering and design tools can facilitate the construction of a completely new biosynthetic pathway. C1 [Siegel, Justin B.] Univ Calif Davis, Dept Chem, Davis, CA 95616 USA. [Siegel, Justin B.] Univ Calif Davis, Dept Biochem & Mol Med, Davis, CA 95616 USA. [Siegel, Justin B.] Univ Calif Davis, Genome Ctr, Davis, CA 95616 USA. [Siegel, Justin B.; Wargacki, Adam J.; Louw, Catherine; Eiben, Christopher B.; Gallaher, Jasmine L.; Bale, Jacob; Yoshikuni, Yasuo; Gelb, Michael H.; Baker, David] Univ Washington, Dept Biochem, Seattle, WA 98195 USA. [Siegel, Justin B.; Wargacki, Adam J.; Louw, Catherine; Eiben, Christopher B.; Gallaher, Jasmine L.; Bale, Jacob; Yoshikuni, Yasuo; Gelb, Michael H.; Baker, David] Univ Washington, Inst Prot Design, Seattle, WA 98195 USA. [Siegel, Justin B.; Baker, David] Univ Washington, Biomol Struct & Design Program, Seattle, WA 98195 USA. [Smith, Amanda Lee; Lidstrom, Mary E.] Univ Washington, Dept Chem Engn, Seattle, WA 98195 USA. [Noor, Elad; Bale, Jacob] Univ Washington, Grad Program Mol & Cellular Biol, Seattle, WA 98195 USA. [Yoshikuni, Yasuo; Baker, David] Univ Washington, Howard Hughes Med Inst, Seattle, WA 98195 USA. [Gelb, Michael H.] Univ Washington, Dept Chem, Seattle, WA 98195 USA. [Lidstrom, Mary E.] Univ Washington, Dept Microbiol, Seattle, WA 98195 USA. [Poust, Sean; Eiben, Christopher B.; Keasling, Jay D.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94270 USA. [Keasling, Jay D.] Univ Calif Berkeley, Inst QB3, Berkeley, CA 94270 USA. [Poust, Sean; Eiben, Christopher B.; Tran, Huu M.; Keasling, Jay D.] Joint BioEnergy Inst, Emeryville, CA 94608 USA. [Bar-Even, Arren; Noor, Elad] Weizmann Inst Sci, Dept Plant Sci, IL-76100 Rehovot, Israel. [Shen, Betty W.; Stoddard, Barry L.] Fred Hutchinson Canc Res Ctr, Div Basic Sci, Seattle, WA 98109 USA. [Tran, Huu M.] Sandia Natl Labs, Biomass Sci & Convers Technol, Livermore, CA 94550 USA. [Yoshikuni, Yasuo] Lawrence Berkeley Natl Lab, Joint Genome Inst, Dept Energy, Walnut Creek, CA 94598 USA. [Keasling, Jay D.] Synthet Biol Engn Res Ctr, Emeryville, CA 94608 USA. [Keasling, Jay D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Lidstrom, ME (reprint author), Univ Washington, Dept Chem Engn, Seattle, WA 98195 USA. EM lidstrom@u.washington.edu; dabaker@uw.edu OI Bale, Jacob/0000-0003-2444-5875; Bar-Even, Arren/0000-0002-1039-4328 FU Advanced Research Projects Agency-Energy [DE-AR0000091]; Joint BioEnergy Institute - Office of Science, Office of Biological and Environmental Research of the US Department of Energy [DE-AC02-05CH11231]; National Institutes of Health [R01 GM498578]; National Science Foundation (NSF) Integrative Graduate Education and Research Traineeship Grant Graduate Education [(DGE)-0654252]; NSF Graduate Research Fellowships Program [DGE 1106400, DGE 0718124]; Howard Hughes Medical Institute FX We thank Olga Khersonsky, Christy Tinberg, Matthew Harger, Janet Matsen, Nick Chavkin, and Curt Fischer, and Jason Kelley of Ginkgo Bioworks for assistance. This work was supported by Advanced Research Projects Agency-Energy Project DE-AR0000091; the Joint BioEnergy Institute, which is funded by the Office of Science, Office of Biological and Environmental Research of the US Department of Energy (Contract DE-AC02-05CH11231); National Institutes of Health Grant R01 GM498578 (to B.W.S. and B.L.S.); National Science Foundation (NSF) Integrative Graduate Education and Research Traineeship Grant Graduate Education (DGE)-0654252 (to A.L.S.); NSF Graduate Research Fellowships Program Grants DGE 1106400 (to S.P.) and DGE 0718124 (to J.B.); and the Howard Hughes Medical Institute (D.B.). NR 38 TC 31 Z9 31 U1 14 U2 66 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAR 24 PY 2015 VL 112 IS 12 BP 3704 EP 3709 DI 10.1073/pnas.1500545112 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CE0EJ UT WOS:000351477000044 PM 25775555 ER PT J AU Koven, CD Lawrence, DM Riley, WJ AF Koven, Charles D. Lawrence, David M. Riley, William J. TI Permafrost carbon-climate feedback is sensitive to deep soil carbon decomposability but not deep soil nitrogen dynamics SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE carbon cycle; Earth system models; cryosphere; soil organic matter; permafrost thaw ID ORGANIC-MATTER; TUNDRA; THAW; BALANCE; FOREST; CO2; ECOSYSTEMS; VEGETATION; EMISSIONS; TURNOVER AB Permafrost soils contain enormous amounts of organic carbon whose stability is contingent on remaining frozen. With future warming, these soils may release carbon to the atmosphere and act as a positive feedback to climate change. Significant uncertainty remains on the postthaw carbon dynamics of permafrost-affected ecosystems, in particular since most of the carbon resides at depth where decomposition dynamics may differ from surface soils, and since nitrogen mineralized by decomposition may enhance plant growth. Here we show, using a carbon-nitrogen model that includes permafrost processes forced in an unmitigated warming scenario, that the future carbon balance of the permafrost region is highly sensitive to the decomposability of deeper carbon, with the net balance ranging from 21 Pg C to 164 Pg C losses by 2300. Increased soil nitrogen mineralization reduces nutrient limitations, but the impact of deep nitrogen on the carbon budget is small due to enhanced nitrogen availability from warming surface soils and seasonal asynchrony between deeper nitrogen availability and plant nitrogen demands. Although nitrogen dynamics are highly uncertain, the future carbon balance of this region is projected to hinge more on the rate and extent of permafrost thaw and soil decomposition than on enhanced nitrogen availability for vegetation growth resulting from permafrost thaw. C1 [Koven, Charles D.; Riley, William J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Lawrence, David M.] Natl Ctr Atmospher Res, Climate & Global Dynam Div, Boulder, CO 80305 USA. RP Koven, CD (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. EM cdkoven@lbl.gov RI Riley, William/D-3345-2015; Lawrence, David/C-4026-2011; Koven, Charles/N-8888-2014 OI Riley, William/0000-0002-4615-2304; Lawrence, David/0000-0002-2968-3023; Koven, Charles/0000-0002-3367-0065 FU Office of Science, Office of Biological and Environmental Research of the US Department of Energy (DOE), Earth System Modeling, Regional and Global Climate Modeling, and Terrestrial Ecosystem Science Programs [DE-AC02-05CH11231]; Office of Science of the US Department of Energy [DE-AC02-05CH11231]; Office of Biological and Environmental Research in the DOE Office of Science; National Science Foundation (NSF); NSF [AGS-1048996, ARC-1048987]; Office of Science (BER) of the US Department of Energy; US Department of Energy BER, as part of its Climate Change Prediction Program [DE-FC03-97ER62402/A010] FX This research was supported by the Director, Office of Science, Office of Biological and Environmental Research of the US Department of Energy (DOE) under Contract DE-AC02-05CH11231 as part of their Earth System Modeling, Regional and Global Climate Modeling, and Terrestrial Ecosystem Science Programs and used resources of the National Energy Research Scientific Computing Center, also supported by the Office of Science of the US Department of Energy, under Contract DE-AC02-05CH11231. The Next-Generation Ecosystem Experiments (NGEE Arctic) project is supported by the Office of Biological and Environmental Research in the DOE Office of Science. National Center for Atmospheric Research (NCAR) is sponsored by the National Science Foundation (NSF). The CESM project is supported by the NSF and the Office of Science (BER) of the US Department of Energy. Computing resources were provided by the Climate Simulation Laboratory at NCAR's Computational and Information Systems Laboratory, sponsored by NSF and other agencies. D.M.L. is supported by funding from the US Department of Energy BER, as part of its Climate Change Prediction Program, Cooperative Agreement DE-FC03-97ER62402/A010 and NSF Grants AGS-1048996 and ARC-1048987. NR 47 TC 31 Z9 32 U1 26 U2 97 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAR 24 PY 2015 VL 112 IS 12 BP 3752 EP 3757 DI 10.1073/pnas.1415123112 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CE0EJ UT WOS:000351477000052 PM 25775603 ER PT J AU Piotrowski, JS Okada, H Lu, FC Li, SC Hinchman, L Ranjan, A Smith, DL Higbee, AJ Ulbrich, A Coon, JJ Deshpande, R Bukhman, YV McIlwain, S Ong, IM Myers, CL Boone, C Landick, R Ralph, J Kabbage, M Ohya, Y AF Piotrowski, Jeff S. Okada, Hiroki Lu, Fachuang Li, Sheena C. Hinchman, Li Ranjan, Ashish Smith, Damon L. Higbee, Alan J. Ulbrich, Arne Coon, Joshua J. Deshpande, Raamesh Bukhman, Yury V. McIlwain, Sean Ong, Irene M. Myers, Chad L. Boone, Charles Landick, Robert Ralph, John Kabbage, Mehdi Ohya, Yoshikazu TI Plant-derived antifungal agent poacic acid targets beta-1,3-glucan SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE chemical genomics; high-dimensional morphometrics; lignocellulosic hydrolysates; fungal cell wall; Saccharomyces cerevisiae ID YEAST 1,3-BETA-GLUCAN SYNTHASE; CELL-WALL BIOGENESIS; SACCHAROMYCES-CEREVISIAE; LIGNOCELLULOSIC MATERIALS; ENDOPLASMIC-RETICULUM; ETHANOL-PRODUCTION; INTEGRITY PATHWAY; CANDIDA-ALBICANS; DRUG CASPOFUNGIN; CLIMATE-CHANGE AB A rise in resistance to current antifungals necessitates strategies to identify alternative sources of effective fungicides. We report the discovery of poacic acid, a potent antifungal compound found in lignocellulosic hydrolysates of grasses. Chemical genomics using Saccharomyces cerevisiae showed that loss of cell wall synthesis and maintenance genes conferred increased sensitivity to poacic acid. Morphological analysis revealed that cells treated with poacic acid behaved similarly to cells treated with other cell wall-targeting drugs and mutants with deletions in genes involved in processes related to cell wall biogenesis. Poacic acid causes rapid cell lysis and is synergistic with caspofungin and fluconazole. The cellular target was identified; poacic acid localized to the cell wall and inhibited beta-1,3-glucan synthesis in vivo and in vitro, apparently by directly binding beta-1,3-glucan. Through its activity on the glucan layer, poacic acid inhibits growth of the fungi Sclerotinia sclerotiorum and Alternaria solani aswell as the oomycete Phytophthora sojae. A single application of poacic acid to leaves infected with the broadrange fungal pathogen S. sclerotiorum substantially reduced lesion development. The discovery of poacic acid as a natural antifungal agent targeting beta-1,3-glucan highlights the potential side use of products generated in the processing of renewable biomass toward biofuels as a source of valuable bioactive compounds and further clarifies the nature and mechanism of fermentation inhibitors found in lignocellulosic hydrolysates. C1 [Piotrowski, Jeff S.; Lu, Fachuang; Hinchman, Li; Bukhman, Yury V.; McIlwain, Sean; Ong, Irene M.; Landick, Robert; Ralph, John] Univ Wisconsin, Great Lakes Bioenergy Res Ctr, Madison, WI 53703 USA. [Ranjan, Ashish; Smith, Damon L.; Kabbage, Mehdi] Univ Wisconsin, Dept Plant Pathol, Madison, WI 53706 USA. [Higbee, Alan J.; Ulbrich, Arne; Coon, Joshua J.] Univ Wisconsin, Dept Chem, Madison, WI 53703 USA. [Okada, Hiroki; Ohya, Yoshikazu] Univ Tokyo, Grad Sch Frontier Sci, Dept Integrated Biosci, Kashiwa, Chiba 2778561, Japan. [Li, Sheena C.; Boone, Charles] RIKEN, Ctr Sustainable Resource Sci, Wako, Saitama 3510198, Japan. [Deshpande, Raamesh; Myers, Chad L.] Univ Minnesota Twin Cities, Dept Comp Sci & Engn, Minneapolis, MN 55455 USA. [Boone, Charles] Univ Toronto, Terrence Donnelly Ctr Cellular & Biomol Res, Toronto, ON M5S 3E1, Canada. RP Piotrowski, JS (reprint author), Univ Wisconsin, Great Lakes Bioenergy Res Ctr, Madison, WI 53703 USA. EM jpiotrowski@wisc.edu; ohya@k.u-tokyo.ac.jp FU Department of Energy (DOE) Great Lakes Bioenergy Research Center DOE Biological and Environmental Research Office of Science Grant [DE-FC02-07ER64494]; Wisconsin Alumni Research Foundation Award [MSN178899]; RIKEN Foreign Postdoctoral Fellowship; Wisconsin Soybean Marketing Board Grant [MSN172403]; National Institutes of Health [1R01HG005084-01A1, 1R01GM104975-01, R01HG005853]; National Science Foundation Grant [DBI 0953881]; Canadian Institute for Advanced Research Genetic Networks Program; United Soybean Board Grant [MSN143317]; Ministry of Education, Culture, Sports, Science and Technology, Japan [24370002] FX We thank T. K. Sato, E. Hendel, S. Morford, and N. Keller for critical discussions of the manuscript. J.S.P., F.L., L.H., A.J.H., A.U., J.J.C., S.M., I.M.O., and J.R. are funded by Department of Energy (DOE) Great Lakes Bioenergy Research Center DOE Biological and Environmental Research Office of Science Grant DE-FC02-07ER64494. J.S.P., F.L., and M.K. are supported by Wisconsin Alumni Research Foundation Award MSN178899. H.O. is a research fellow of the Japan Society for the Promotion of Science. S.C.L. is supported by a RIKEN Foreign Postdoctoral Fellowship. A.R., D.L.S., and M.K. are supported by Wisconsin Soybean Marketing Board Grant MSN172403. R.D. and C.L.M. are supported by National Institutes of Health Grants 1R01HG005084-01A1, 1R01GM104975-01, and R01HG005853 and National Science Foundation Grant DBI 0953881. C.L.M. and C.B. are supported by the Canadian Institute for Advanced Research Genetic Networks Program. M.K. is supported by United Soybean Board Grant MSN143317. Y.O. is supported by Ministry of Education, Culture, Sports, Science and Technology, Japan Grant for Scientific Research 24370002. NR 61 TC 7 Z9 7 U1 9 U2 52 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAR 24 PY 2015 VL 112 IS 12 BP E1490 EP E1497 DI 10.1073/pnas.1410400112 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CE0EJ UT WOS:000351477000014 PM 25775513 ER PT J AU Park, Y Choi, JS Choi, T Lee, MJ Jia, Q Park, M Lee, H Park, BH AF Park, Yeonggu Choi, Jin Sik Choi, Taekjib Lee, Mi Jung Jia, Quanxi Park, Minwoo Lee, Hoonkyung Park, Bae Ho TI Configuration of ripple domains and their topological defects formed under local mechanical stress on hexagonal monolayer graphene SO SCIENTIFIC REPORTS LA English DT Article ID ATOMIC-SCALE; ANNIHILATION; ORIENTATION; DISLOCATION; MEMBRANES; VORTICES; FILMS; WATER AB Ripples in graphene are extensively investigated because they ensure the mechanical stability of two-dimensional graphene and affect its electronic properties. They arise from spontaneous symmetry breaking and are usually manifested in the form of domains with long-range order. It is expected that topological defects accompany a material exhibiting long-range order, whose functionality depends on characteristics of domains and topological defects. However, there remains a lack of understanding regarding ripple domains and their topological defects formed on monolayer graphene. Here we explore configuration of ripple domains and their topological defects in exfoliated monolayer graphenes on SiO2/Si substrates using transverse shear microscope. We observe three-color domains with three different ripple directions, which meet at a core. Furthermore, the closed domain is surrounded by an even number of cores connected together by domain boundaries, similar to topological vortex and anti-vortex pairs. In addition, we have found that axisymmetric three-color domains can be induced around nanoparticles underneath the graphene. This fascinating configuration of ripple domains may result from the intrinsic hexagonal symmetry of two-dimensional graphene, which is supported by theoretical simulation using molecular dynamics. Our findings are expected to play a key role in understanding of ripple physics in graphene and other two-dimensional materials. C1 [Park, Yeonggu; Lee, Mi Jung; Jia, Quanxi; Park, Minwoo; Lee, Hoonkyung; Park, Bae Ho] Konkuk Univ, Dept Phys, Div Quantum Phases & Devices, Seoul 143701, South Korea. [Choi, Jin Sik] Elect & Telecommun Res Inst, Creat Res Ctr Graphene Elect, Taejon 305700, South Korea. [Choi, Taekjib] Sejong Univ, Dept Nanotechnol & Adv Mat Engn, Hybrid Mat Res Ctr, Seoul 143747, South Korea. [Jia, Quanxi] Los Alamos Natl Lab, Ctr Integrated Nanotechnol CINT, Los Alamos, NM 87545 USA. RP Park, BH (reprint author), Konkuk Univ, Dept Phys, Div Quantum Phases & Devices, Seoul 143701, South Korea. EM baehpark@konkuk.ac.kr RI Choi, Taekjib/H-8791-2012 OI Choi, Taekjib/0000-0001-6912-3322 FU National Research Foundation of Korea (NRF) - Korea government (MSIP) [2013R1A3A2042120, 2011-0030229, 2014R1A1A1006405, 2012R1A1A1013124]; Creative Research Program of the ETRI of Korea [14ZE1110] FX This work was supported by the National Research Foundation of Korea (NRF) grants funded by the Korea government (MSIP) (No. 2013R1A3A2042120, 2011-0030229, 2014R1A1A1006405, and 2012R1A1A1013124). J.S.C. acknowledges the Creative Research Program of the ETRI (14ZE1110) of Korea. We thank H. Kim for help with micro-Raman spectroscopy. NR 32 TC 0 Z9 0 U1 5 U2 50 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAR 24 PY 2015 VL 5 AR 9390 DI 10.1038/srep09390 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CE3BY UT WOS:000351700500001 PM 25801337 ER PT J AU Zhou, Y Han, ST Sonar, P Ma, XL Chen, JH Zheng, ZJ Roy, VAL AF Zhou, Ye Han, Su-Ting Sonar, Prashant Ma, Xinlei Chen, Jihua Zheng, Zijian Roy, V. A. L. TI Reversible Conversion of Dominant Polarity in Ambipolar Polymer/Graphene Oxide Hybrids SO SCIENTIFIC REPORTS LA English DT Article ID FIELD-EFFECT TRANSISTORS; THIN-FILM TRANSISTORS; HIGH-PERFORMANCE; CHARGE INJECTION; GRAPHENE OXIDE; POLYMER SEMICONDUCTORS; INTEGRATED-CIRCUITS; CONJUGATED-POLYMER; MOBILITY; TRANSPORT AB The possibility to selectively modulate the charge carrier transport in semiconducting materials is extremely challenging for the development of high performance and low-power consuming logic circuits. Systematical control over the polarity (electrons and holes) in transistor based on solution processed layer by layer polymer/graphene oxide hybrid system has been demonstrated. The conversion degree of the polarity is well controlled and reversible by trapping the opposite carriers. Basically, an electron device is switched to be a hole only device or vice versa. Finally, a hybrid layer ambipolar inverter is demonstrated in which almost no leakage of opposite carrier is found. This hybrid material has wide range of applications in planar p-n junctions and logic circuits for high-throughput manufacturing of printed electronic circuits. C1 [Zhou, Ye; Han, Su-Ting; Roy, V. A. L.] City Univ Hong Kong, Dept Phys & Mat Sci, Kowloon Tong, Hong Kong, Peoples R China. [Sonar, Prashant] QUT, Sch Chem Phys & Mech Engn, Brisbane, Qld 4001, Australia. [Ma, Xinlei; Zheng, Zijian] Hong Kong Polytech Univ, Inst Text & Clothing, Nanotechnol Ctr, Kowloon, Hong Kong, Peoples R China. [Chen, Jihua] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Roy, V. A. L.] City Univ Hong Kong, Shenzhen Res Inst, Shenzhen 518057, Peoples R China. RP Roy, VAL (reprint author), City Univ Hong Kong, Dept Phys & Mat Sci, Tat Chee Ave, Kowloon Tong, Hong Kong, Peoples R China. EM val.roy@cityu.edu.hk RI Chen, Jihua/F-1417-2011; Zhou, Ye/G-8328-2012; ZHENG, ZIJIAN/B-4012-2009; OI Chen, Jihua/0000-0001-6879-5936; Zhou, Ye/0000-0002-0273-007X; ZHENG, ZIJIAN/0000-0002-6653-7594; VELLAISAMY, Arul Lenus Roy/0000-0003-1432-9950; Sonar, Prashant/0000-0002-1119-4897 FU City University of Hong Kong's Strategic Research Grant [7004012]; Research Grants Council of the Hong Kong Special Administrative Region [T23-713/11]; Shenzhen Municipality project [JCYJ20120618115445056]; Division of Scientific User Facilities, Office of Basic Energy Sciences, U.S. Department of Energy FX We acknowledge grants from City University of Hong Kong's Strategic Research Grant Project no. 7004012, the Research Grants Council of the Hong Kong Special Administrative Region (Project No. T23-713/11) and Shenzhen Municipality project no. JCYJ20120618115445056. TEM and electron diffraction were conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Division of Scientific User Facilities, Office of Basic Energy Sciences, U.S. Department of Energy. NR 62 TC 5 Z9 5 U1 6 U2 47 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAR 24 PY 2015 VL 5 AR 9446 DI 10.1038/srep09446 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CE3CT UT WOS:000351702800001 PM 25801827 ER PT J AU Kiani, S Ratsch, C Minor, AM Kodambaka, S Yang, JM AF Kiani, S. Ratsch, C. Minor, A. M. Kodambaka, S. Yang, J. -M. TI Orientation- and size-dependent room-temperature plasticity in ZrC crystals SO PHILOSOPHICAL MAGAZINE LA English DT Article DE plasticity; carbides; microscopy ID TO-DUCTILE TRANSITION; TITANIUM CARBIDE; SINGLE-CRYSTALS; DEFORMATION MECHANISMS; STRUCTURAL CERAMICS; HARDNESS ANISOTROPY; CUBIC CARBIDES; COMPRESSION; SILICON; BEHAVIOR AB Using in situ electron microscopy-based nanomechanical testing, we show that sub-micron-scale ZrC(100) and ZrC(111) single crystals exhibit size- and orientation-dependent room-temperature plasticity under compression. We identify { [GRAPHICS] } [GRAPHICS] and {0 0 1} [GRAPHICS] as the active slip systems operating in ZrC(100) and ZrC(111) crystals, respectively. For both the orientations, yield strengths increase with decreasing crystal size. ZrC(111) is found to be up to 10x softer than ZrC(100). Using density functional theory calculations, we attribute the observed anisotropy to surprisingly facile shear along {0 0 1} [GRAPHICS] compared to { [GRAPHICS] } [GRAPHICS] . Based upon our results, which provide important insights into plastic deformation modes operating in ZrC, we expect that slip systems other than { [GRAPHICS] } [GRAPHICS] can be softer and operate at low temperatures in NaCl-structured refractory transition-metal carbides and nitrides. C1 [Kiani, S.; Kodambaka, S.; Yang, J. -M.] Univ Calif Los Angeles, Dept Mat Sci & Engn, Los Angeles, CA 90095 USA. [Ratsch, C.] Univ Calif Los Angeles, Dept Math, Los Angeles, CA 90095 USA. [Ratsch, C.] Univ Calif Los Angeles, Inst Pure & Appl Math, Los Angeles, CA 90095 USA. [Minor, A. M.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Minor, A. M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Natl Ctr Electron Microscopy, Berkeley, CA 94720 USA. RP Kodambaka, S (reprint author), Univ Calif Los Angeles, Dept Mat Sci & Engn, Los Angeles, CA 90095 USA. EM kodambaka@ucla.edu; jyang@seas.ucla.edu RI Foundry, Molecular/G-9968-2014 FU Air Force Office of Scientific Research [FA9550-10-1-0496]; National Science Foundation [DMS-0931852]; Office of Science, Office of Basic Energy Sciences, of the US Department of Energy [DE-AC02-05CH11231] FX SK and JMY are thankful for the funding from the Air Force Office of Scientific Research (Dr Ali Sayir) [grant number FA9550-10-1-0496]. CR gratefully acknowledges support from National Science Foundation [grant number DMS-0931852]. The in situ electron microscopy experiments are conducted as part of a user project at the National Center for Electron Microscopy, Lawrence Berkeley National Laboratory, supported by the Office of Science, Office of Basic Energy Sciences, of the US Department of Energy [grant number DE-AC02-05CH11231]. NR 48 TC 2 Z9 2 U1 4 U2 21 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND SN 1478-6435 EI 1478-6443 J9 PHILOS MAG JI Philos. Mag. PD MAR 24 PY 2015 VL 95 IS 9 BP 985 EP 997 DI 10.1080/14786435.2015.1012568 PG 13 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering; Physics, Applied; Physics, Condensed Matter SC Materials Science; Metallurgy & Metallurgical Engineering; Physics GA CD2EN UT WOS:000350887200004 ER PT J AU Sayer, RA AF Sayer, Robert A. TI Generalized Procedure for Improved Accuracy of Thermal Contact Resistance Measurements for Materials With Arbitrary Temperature-Dependent Thermal Conductivity SO HEAT TRANSFER ENGINEERING LA English DT Article ID CARBON-NANOTUBE COMPOSITES; HEAT-TRANSFER; FLOW AB Thermal contact resistance (TCR) is most commonly measured using one-dimensional steady-state calorimetric techniques. In these experimental methods, a temperature gradient is applied across two contacting beams and the temperature drop at the interface is inferred from the temperature profiles of the rods that are measured at discrete points. During data analysis, thermal conductivity of the beams is typically taken to be an average value over the temperature range imposed during the experiment. Here, a generalized theory is presented that accounts for temperature-dependent changes in thermal conductivity. The procedure presented enables accurate measurement of TCR for contacting materials whose thermal conductivity is any arbitrary function of temperature. For example, it is shown that the standard technique yields TCR values that are about 15% below the actual value for two specific examples of copper and silicon contacts. On the other hand, the generalized technique predicts TCR values that are within 1% of the actual value. The method is exact when thermal conductivity is known exactly and no other errors are introduced to the system. C1 Sandia Natl Labs, Engn Sci Ctr, Albuquerque, NM 87185 USA. RP Sayer, RA (reprint author), Sandia Natl Labs, Engn Sci Ctr, POB 5800, Albuquerque, NM 87185 USA. EM rsayer@sandia.gov FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 23 TC 0 Z9 0 U1 1 U2 41 PU TAYLOR & FRANCIS INC PI PHILADELPHIA PA 530 WALNUT STREET, STE 850, PHILADELPHIA, PA 19106 USA SN 0145-7632 EI 1521-0537 J9 HEAT TRANSFER ENG JI Heat Transf. Eng. PD MAR 24 PY 2015 VL 36 IS 5 BP 433 EP 438 DI 10.1080/01457632.2014.932553 PG 6 WC Thermodynamics; Engineering, Mechanical; Mechanics SC Thermodynamics; Engineering; Mechanics GA AR5UJ UT WOS:000343648900001 ER PT J AU Chung, D Young, J Bomble, YJ Vander Wall, TA Groom, J Himmel, ME Westpheling, J AF Chung, Daehwan Young, Jenna Bomble, Yannick J. Vander Wall, Todd A. Groom, Joseph Himmel, Michael E. Westpheling, Janet TI Homologous Expression of the Caldicellulosiruptor bescii CelA Reveals that the Extracellular Protein Is Glycosylated SO PLOS ONE LA English DT Article ID STREPTOMYCES-LIVIDANS GLYCOSYLATES; CARBOHYDRATE-BINDING MODULE; ACCESSORY SEC SYSTEM; CELLULOMONAS-FIMI; STREPTOCOCCUS-GORDONII; MUTATIONAL ANALYSIS; PICHIA-PASTORIS; PLANT BIOMASS; GLYCOPROTEINS; DELETION AB Members of the bacterial genus Caldicellulosiruptor are the most thermophilic cellulolytic microbes described with ability to digest lignocellulosic biomass without conventional pretreatment. The cellulolytic ability of different species varies dramatically and correlates with the presence of the multimodular cellulase CelA, which contains both a glycoside hydrolase family 9 endoglucanase and a glycoside hydrolase family 48 exoglucanase known to be synergistic in their activity, connected by three cellulose-binding domains via linker peptides. This architecture exploits the cellulose surface ablation driven by its general cellulase processivity as well as excavates cavities into the surface of the substrate, revealing a novel paradigm for cellulase activity. We recently reported that a deletion of celA in C. bescii had a significant effect on its ability to utilize complex biomass. To analyze the structure and function of CelA and its role in biomass deconstruction, we constructed a new expression vector for C. bescii and were able, for the first time, to express significant quantities of full-length protein in vivo in the native host. The protein, which contains a Histidine tag, was active and excreted from the cell. Expression of CelA protein with and without its signal sequence allowed comparison of protein retained intracellularly to protein transported extra-cellularly. Analysis of protein in culture supernatants revealed that the extracellular CelA protein is glycosylated whereas the intracellular CelA is not, suggesting that either protein transport is required for this post-translational modification or that glycosylation is required for protein export. The mechanism and role of protein glycosylation in bacteria is poorly understood and the ability to express CelA in vivo in C. bescii will allow the study of the mechanism of protein glycosylation in this thermophile. It will also allow the study of glycosylation of CelA itself and its role in the structure and function of this important enzyme in biomass deconstruction. C1 [Chung, Daehwan; Young, Jenna; Groom, Joseph; Westpheling, Janet] Univ Georgia, Dept Genet, Athens, GA 30602 USA. [Bomble, Yannick J.; Vander Wall, Todd A.; Himmel, Michael E.] Natl Renewable Energy Lab, Biosci Ctr, Golden, CO USA. [Chung, Daehwan; Young, Jenna; Bomble, Yannick J.; Vander Wall, Todd A.; Groom, Joseph; Himmel, Michael E.; Westpheling, Janet] Oak Ridge Natl Lab, BioEnergy Sci Ctr, Oak Ridge, TN USA. RP Westpheling, J (reprint author), Univ Georgia, Dept Genet, Athens, GA 30602 USA. EM janwest@uga.edu FU Office of Biological and Environmental Research in the DOE Office of Science [10-21-RR093-367] FX The BioEnergy Science Center is a U.S. Department of Energy Bioenergy Research Center supported by the Office of Biological and Environmental Research in the DOE Office of Science, grant # 10-21-RR093-367. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 38 TC 5 Z9 6 U1 0 U2 23 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAR 23 PY 2015 VL 10 IS 3 AR UNSP e0119508 DI 10.1371/journal.pone.0119508 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CE6ZS UT WOS:000351987300056 PM 25799047 ER PT J AU Stram, DO Preston, DL Sokolnikov, M Napier, B Kopecky, KJ Boice, J Beck, H Till, J Bouville, A AF Stram, Daniel O. Preston, Dale L. Sokolnikov, Mikhail Napier, Bruce Kopecky, Kenneth J. Boice, John Beck, Harold Till, John Bouville, Andre TI Shared Dosimetry Error in Epidemiological Dose-Response Analyses SO PLOS ONE LA English DT Article ID ATOMIC-BOMB SURVIVORS; ESTIMATING UNCERTAINTY; LUNG-CANCER; RADIATION; REGRESSION; DISEASE; COHORT; RISK; METHODOLOGY; LIKELIHOOD AB Radiation dose reconstruction systems for large-scale epidemiological studies are sophisticated both in providing estimates of dose and in representing dosimetry uncertainty. For example, a computer program was used by the Hanford Thyroid Disease Study to provide 100 realizations of possible dose to study participants. The variation in realizations reflected the range of possible dose for each cohort member consistent with the data on dose determinates in the cohort. Another example is the Mayak Worker Dosimetry System 2013 which estimates both external and internal exposures and provides multiple realizations of "possible" dose history to workers given dose determinants. This paper takes up the problem of dealing with complex dosimetry systems that provide multiple realizations of dose in an epidemiologic analysis. In this paper we derive expected scores and the information matrix for a model used widely in radiation epidemiology, namely the linear excess relative risk (ERR) model that allows for a linear dose response (risk in relation to radiation) and distinguishes between modifiers of background rates and of the excess risk due to exposure. We show that treating the mean dose for each individual (calculated by averaging over the realizations) as if it was true dose (ignoring both shared and unshared dosimetry errors) gives asymptotically unbiased estimates (i.e. the score has expectation zero) and valid tests of the null hypothesis that the ERR slope beta is zero. Although the score is unbiased the information matrix (and hence the standard errors of the estimate of beta) is biased for beta not equal 0 when ignoring errors in dose estimates, and we show how to adjust the information matrix to remove this bias, using the multiple realizations of dose. The use of these methods in the context of several studies including, the Mayak Worker Cohort, and the U.S. Atomic Veterans Study, is discussed. C1 [Stram, Daniel O.] Univ So Calif, Dept Prevent Med, Los Angeles, CA 90089 USA. [Preston, Dale L.] Hirosoft Int, Eureka, CA USA. [Sokolnikov, Mikhail] Southern Urals Biophys Inst, Ozersk, Russia. [Napier, Bruce] Pacific NW Natl Lab, Richland, WA 99352 USA. [Kopecky, Kenneth J.] Fred Hutchinson Canc Ctr, Seattle, WA USA. [Boice, John] Vanderbilt Univ, Nashville, TN 37235 USA. [Beck, Harold] US DOE, New York, NY USA. [Till, John] Risk Assessment Corp, Neeses, SC USA. [Bouville, Andre] NCI, Radiat Epidemiol Branch, Rockville, MD USA. RP Stram, DO (reprint author), Univ So Calif, Dept Prevent Med, Los Angeles, CA 90089 USA. EM Daniel.Stram@med.usc.edu FU National Cancer Institute [U01 CA137026]; U.S. Department of Energy [DE-HS0000091, DE-SC0008944 (doe.gov)]; Discovery Grant from the Vanderbilt-Ingram Cancer Center [404-357-9682 (vicc.org)] FX This research was supported in part by contracts and grants from the National Cancer Institute (grant no. U01 CA137026) (www.cancer.gov), the U.S. Department of Energy (grant nos. DE-HS0000091, and DE-SC0008944) (doe.gov) and a Discovery Grant from the Vanderbilt-Ingram Cancer Center (Center no. 404-357-9682) (vicc.org). Risk Assessment Corporation and Hirosoft International provided support in the form of salaries for authors [JT and DP], but did not have any additional role in the study design, data collection and analysis, decision to publish, or preparation of the manuscript. The specific roles of these authors are articulated in the "author contributions" section. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 38 TC 6 Z9 6 U1 1 U2 4 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAR 23 PY 2015 VL 10 IS 3 AR e0119418 DI 10.1371/journal.pone.0119418 PG 18 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CE6ZS UT WOS:000351987300048 PM 25799311 ER PT J AU Arion, T Neppl, S Roth, F Shavorskiy, A Bluhm, H Hussain, Z Gessner, O Eberhardt, W AF Arion, Tiberiu Neppl, Stefan Roth, Friedrich Shavorskiy, Andrey Bluhm, Hendrik Hussain, Zahid Gessner, Oliver Eberhardt, Wolfgang TI Site-specific probing of charge transfer dynamics in organic photovoltaics SO APPLIED PHYSICS LETTERS LA English DT Article ID ENERGY-LEVEL ALIGNMENT; COPPER PHTHALOCYANINE; ELECTRONIC-STRUCTURE; PHOTOELECTRON-SPECTROSCOPY; CONDUCTING POLYMER; THIN-FILMS; INTERFACE; ABSORPTION; C-60; BUCKMINSTERFULLERENE AB We report the site-specific probing of charge-transfer dynamics in a prototype system for organic photovoltaics (OPVs) by picosecond time-resolved X-ray photoelectron spectroscopy. A layered system consisting of approximately two monolayers of C-60 deposited on top of a thin film of Copper-Phthalocyanine (CuPC) is excited by an optical pump pulse and the induced electronic dynamics are probed with 590 eV X-ray pulses. Charge transfer from the electron donor (CuPC) to the acceptor (C-60) and subsequent charge carrier dynamics are monitored by recording the time-dependent C 1s core level photoemission spectrum of the system. The arrival of electrons in the C-60 layer is readily observed as a completely reversible, transient shift of the C-60 associated C 1s core level, while the C 1s level of the CuPC remains unchanged. The capability to probe charge transfer and recombination dynamics in OPV assemblies directly in the time domain and from the perspective of well-defined domains is expected to open additional pathways to better understand and optimize the performance of this emerging technology. (C) 2015 AIP Publishing LLC. C1 [Arion, Tiberiu; Roth, Friedrich; Eberhardt, Wolfgang] Ctr Free Electron Laser Sci DESY, D-22607 Hamburg, Germany. [Neppl, Stefan; Shavorskiy, Andrey; Bluhm, Hendrik; Gessner, Oliver] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Hussain, Zahid; Eberhardt, Wolfgang] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, ALS, Berkeley, CA 94720 USA. [Eberhardt, Wolfgang] Tech Univ Berlin, Inst Opt & Atom Phys, D-10623 Berlin, Germany. RP Arion, T (reprint author), Ctr Free Electron Laser Sci DESY, Notkestr 85, D-22607 Hamburg, Germany. RI Roth, Friedrich/J-3084-2015 FU Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; Office of Science of the U.S. Department of Energy at the Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; Office of Basic Energy Sciencesof the U.S. Department of Energy at the Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; Division of Chemical Sciences, Geosciences, and Biosciences of the U.S. Department of Energy at the Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; ALS FX Fruitful discussions with D. S. Pemmaraju are gratefully acknowledged. We acknowledge the allocation of beam time at the beam line 11.0.2. of the ALS, as well as the support of the ALS staff during the beam time. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The Molecular Environmental Sciences beamline 11.0.2 is supported by the Director, Office of Science, Office of Basic Energy Sciences, and the Division of Chemical Sciences, Geosciences, and Biosciences of the U.S. Department of Energy at the Lawrence Berkeley National Laboratory under Contract No. DE-AC02-05CH11231. One of us (W.E.) would like to thank the ALS for their support and hospitality. O.G. was supported by the Department of Energy Office of Science Early Career Research Program. S.N. acknowledges support by the Alexander von Humboldt foundation. NR 32 TC 3 Z9 3 U1 1 U2 28 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAR 23 PY 2015 VL 106 IS 12 AR 121602 DI 10.1063/1.4916278 PG 5 WC Physics, Applied SC Physics GA CE5LM UT WOS:000351876700014 ER PT J AU Bisig, A Mawass, MA Stark, M Moutafis, C Rhensius, J Heidler, J Gliga, S Weigand, M Tyliszczak, T Van Waeyenberge, B Stoll, H Schutz, G Klaui, M AF Bisig, Andre Mawass, Mohamad-Assaad Staerk, Martin Moutafis, Christoforos Rhensius, Jan Heidler, Jakoba Gliga, Sebastian Weigand, Markus Tyliszczak, Tolek Van Waeyenberge, Bartel Stoll, Hermann Schuetz, Gisela Klaeui, Mathias TI Dynamic domain wall chirality rectification by rotating magnetic fields SO APPLIED PHYSICS LETTERS LA English DT Article ID SPIN STRUCTURE; STATE; STRIPS; MOTION AB We report on the observation of magnetic vortex domain wall chirality reversal in ferromagnetic rings that is controlled by the sense of rotation of a magnetic field. We use time-resolved X-ray microscopy to dynamically image the chirality-switching process and perform micromagnetic simulations to deduce the switching details from time-resolved snapshots. We find experimentally that the switching occurs within less than 4 ns and is observed in all samples with ring widths ranging from 0.5 mu m to 2 mu m, ring diameters between 2 mu m and 5 mu m, and a thickness of 30 nm, where a vortex domain wall is present in the magnetic onion state of the ring. From the magnetic contrast in the time-resolved images, we can identify effects of thermal activation, which plays a role for the switching process. Moreover, we find that the process is highly reproducible so that the domain wall chirality can be set with high fidelity. (C) 2015 AIP Publishing LLC. C1 [Bisig, Andre; Staerk, Martin; Moutafis, Christoforos; Rhensius, Jan; Heidler, Jakoba; Klaeui, Mathias] Univ Konstanz, Dept Phys, D-78457 Constance, Germany. [Bisig, Andre; Mawass, Mohamad-Assaad; Weigand, Markus; Stoll, Hermann; Schuetz, Gisela] Max Planck Inst Intelligent Syst, D-70569 Stuttgart, Germany. [Bisig, Andre; Staerk, Martin; Moutafis, Christoforos; Rhensius, Jan; Heidler, Jakoba; Gliga, Sebastian; Klaeui, Mathias] Paul Scherrer Inst, CH-5232 Villigen, Switzerland. [Bisig, Andre; Staerk, Martin; Moutafis, Christoforos; Heidler, Jakoba; Klaeui, Mathias] Ecole Polytech Fed Lausanne, Inst Condensed Matter Phys, CH-1015 Lausanne, Switzerland. [Bisig, Andre; Mawass, Mohamad-Assaad; Klaeui, Mathias] Johannes Gutenberg Univ Mainz, Inst Phys, D-55099 Mainz, Germany. [Bisig, Andre] IBM Res Zurich, CH-8803 Ruschlikon, Switzerland. [Gliga, Sebastian] ETH, Dept Mat, Lab Mesoscop Syst, CH-8093 Zurich, Switzerland. [Tyliszczak, Tolek] LBNL, Adv Light Source, Berkeley, CA 94720 USA. [Van Waeyenberge, Bartel] Univ Ghent, Dept Solid State Sci, B-9000 Ghent, Belgium. RP Bisig, A (reprint author), Univ Konstanz, Dept Phys, D-78457 Constance, Germany. EM andre.bisig@gmail.com; klaeui@uni-mainz.de RI Klaui, Mathias/B-6972-2009; Gliga, Sebastian/K-4019-2015; EPFL, Physics/O-6514-2016 OI Klaui, Mathias/0000-0002-4848-2569; Gliga, Sebastian/0000-0003-1729-1070; FU German Science Foundation [DFG SFB 767, KL1811, MAINZ GSC 266]; ERC [2007-Stg 208162]; EU [MAGWIRE FP7-ICT-2009-5 257707, SpinIcur FP7-PEOPLE-2012-ITN 316657, WALL FP7-PEOPLE-2013-ITN 608031]; Center for innovative and emerging materials (CINEMA); Swiss National Science Foundation; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX We thank R. Allenspach for helpful discussions. The authors acknowledge support by the German Science Foundation (DFG SFB 767, KL1811, MAINZ GSC 266), the ERC (2007-Stg 208162), the EU (MAGWIRE FP7-ICT-2009-5 257707, SpinIcur FP7-PEOPLE-2012-ITN 316657, WALL FP7-PEOPLE-2013-ITN 608031), the Center for innovative and emerging materials (CINEMA), and the Swiss National Science Foundation. Part of this work was carried out at the MAXYMUS scanning X-ray microscope at HZB, BESSY II in Berlin, Germany. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 37 TC 1 Z9 1 U1 2 U2 37 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAR 23 PY 2015 VL 106 IS 12 AR 122401 DI 10.1063/1.4915256 PG 5 WC Physics, Applied SC Physics GA CE5LM UT WOS:000351876700027 ER PT J AU Sun, JF Mukhopadhyay, S Subedi, A Siegrist, T Singh, DJ AF Sun, Jifeng Mukhopadhyay, Saikat Subedi, Alaska Siegrist, Theo Singh, David J. TI Transport properties of cubic crystalline Ge2Sb2Te5: A potential low-temperature thermoelectric material SO APPLIED PHYSICS LETTERS LA English DT Article ID PHASE-CHANGE MATERIALS; ELECTRONIC-PROPERTIES; LAYERED COMPOUNDS; CONDUCTIVITY; PERFORMANCE; DISORDER; ALLOYS; FILMS; GE; SB AB Ge2Sb2Te5 (GST) has been widely used as a popular phase change material. In this study, we show that it exhibits high Seebeck coefficients 200-300 lV/K in its cubic crystalline phase (c-GST) at remarkably high p-type doping levels of similar to 1 x 10(19)-6 x 10(19) cm(-3) at room temperature. More importantly, at low temperature (T = 200K), the Seebeck coefficient was found to exceed 200 lV/K for a doping range of 1 x 10(19)-3.5 x 10(19) cm(-3). Given that the lattice thermal conductivity in this phase has already been measured to be extremely low (similar to 0.7W/m-K at 300K) [K.S. Siegert et al., Rep. Prog. Phys. 78, 013001 (2015)], our results suggest the possibility of using c-GST as a low-temperature thermoelectric material. (C) 2015 AIP Publishing LLC. C1 [Sun, Jifeng; Mukhopadhyay, Saikat; Singh, David J.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Sun, Jifeng; Siegrist, Theo] Florida Agr & Mech Univ Florida State Univ, Coll Engn, Dept Chem & Biomed Engn, Tallahassee, FL 32310 USA. [Sun, Jifeng; Siegrist, Theo] Natl High Magnet Field Lab, Tallahassee, FL 32310 USA. [Subedi, Alaska] Max Planck Inst Struct & Dynam Matter, Hamburg, Germany. RP Sun, JF (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RI Mukhopadhyay, Saikat/B-4402-2011 FU Department of Energy through the S3TEC energy frontier research center; Department of Energy, Basic Energy Science, Materials Sciences and Engineering Division through the ORNL GO! program FX This work was supported by the Department of Energy through the S3TEC energy frontier research center. J.S. acknowledges a graduate student fellowship, funded by the Department of Energy, Basic Energy Science, Materials Sciences and Engineering Division through the ORNL GO! program. A portion of this work was performed at high-performance computing center at the National High Magnetic Field Laboratory. NR 40 TC 4 Z9 4 U1 8 U2 50 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAR 23 PY 2015 VL 106 IS 12 AR 123907 DI 10.1063/1.4916558 PG 4 WC Physics, Applied SC Physics GA CE5LM UT WOS:000351876700063 ER PT J AU Yang, H Lee, HS Kotula, PG Sato, Y Ikuhara, Y Browning, ND AF Yang, H. Lee, H. S. Kotula, P. G. Sato, Y. Ikuhara, Y. Browning, N. D. TI Amphoteric doping of praseodymium Pr3+ in SrTiO3 grain boundaries SO APPLIED PHYSICS LETTERS LA English DT Article ID PHOTOLUMINESCENCE PROPERTIES; ENERGY; BICRYSTALS; TITANATES; EMISSION; CATIO3; IONS AB Charge compensation in rare-earth Praseodymium (Pr3+) doped SrTiO3 plays an important role in determining the overall photoluminescence properties of the system. Here, the Pr3+ doping behavior in SrTiO3 grain boundaries (GBs) is analyzed using aberration corrected scanning transmission electron microscopy. The presence of Pr3+ induces structural variations and changes the statistical prevalence of the GB structures. In contrast to the assumption that Pr3+ substitutes on the Sr site in the bulk, Pr3+ is found to substitute on both Sr and Ti sites inside the GBs, with the highest concentration at the Ti sites. This amphoteric doping behavior in the boundary plane is further confirmed by first principles theoretical calculations. (C) 2015 AIP Publishing LLC. C1 [Yang, H.] Univ Calif Davis, Davis, CA 95616 USA. [Lee, H. S.] Korean Inst Mat Sci, Chang Won 641831, Gyeongnam, South Korea. [Kotula, P. G.] Sandia Natl Lab Labs, Dept Mat Characterizat, Albuquerque, NM 87123 USA. [Sato, Y.] Kyushu Univ, Dept Mat Sci & Engn, Fukuoka 8190395, Japan. [Ikuhara, Y.] Univ Tokyo, Inst Engn Innovat, Bunkyo Ku, Tokyo 1138656, Japan. [Browning, N. D.] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. RP Yang, H (reprint author), Univ Oxford, Dept Mat, 16 Parks Rd, Oxford OX1 3PH, England. EM haoyang.tem@gmail.com RI Kotula, Paul/A-7657-2011; Ikuhara, Yuichi/N-1001-2015; Ikuhara, Yuichi/F-3066-2010; U-ID, Kyushu/C-5291-2016; OI Kotula, Paul/0000-0002-7521-2759; Ikuhara, Yuichi/0000-0003-3886-005X; Yang, Hao/0000-0003-2326-7317; Browning, Nigel/0000-0003-0491-251X FU United States Department of Energy [DE-FG02-03ER46057]; Ministry of Education, Culture, Sports, Science and Technology (MEXT), Japan; Chemical Imaging Initiative at Pacific Northwest National Laboratory (PNNL) [DE-AC05-76RL01830]; Department of Energy's Office of Biological and Environmental Research; U.S. Department of Energy [DEAC04-94AL85000] FX This work was supported by the United States Department of Energy Grant No. DE-FG02-03ER46057. A part of the work was conducted in the ShaRE user facility at Oak Ridge National Laboratory, and in the Research Hub for Advanced Nano Characterization, The University of Tokyo, supported by the Ministry of Education, Culture, Sports, Science and Technology (MEXT), Japan. A portion of this work was part of the Chemical Imaging Initiative at Pacific Northwest National Laboratory (PNNL) under Contract No. DE-AC05-76RL01830 operated for DOE by Battelle. It was conducted under the Laboratory Directed Research and Development Program at PNNL. A portion of the research was performed using EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at PNNL. A portion of the research was also performed in Sandia National Laboratories. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the U.S. Department of Energy under Contract No. DEAC04-94AL85000. NR 26 TC 1 Z9 1 U1 1 U2 38 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAR 23 PY 2015 VL 106 IS 12 AR 121904 DI 10.1063/1.4916223 PG 5 WC Physics, Applied SC Physics GA CE5LM UT WOS:000351876700019 ER PT J AU Yang, YC Tanaka, K Liu, J Anders, A AF Yang, Yuchen Tanaka, Koichi Liu, Jason Anders, Andre TI Ion energies in high power impulse magnetron sputtering with and without localized ionization zones SO APPLIED PHYSICS LETTERS LA English DT Article ID DISCHARGE; INHOMOGENEITIES; CURRENTS; ATOMS AB High speed imaging of high power impulse magnetron sputtering discharges has revealed that ionization is localized in moving ionization zones but localization disappears at high currents for high yield targets. This offers an opportunity to study the effect ionization zones have on ion energies. We measure that ions have generally higher energies when ionization zones are present, supporting the concept that these zones are associated with moving potential humps. We propose that the disappearance of ionization zones is caused by an increased supply of atoms from the target which cools electrons and reduces depletion of atoms to be ionized. (C) 2015 AIP Publishing LLC. C1 [Yang, Yuchen] Huazhong Univ Sci & Technol, Sch Mat Sci & Engn, State Key Lab Mat Proc & Die & Mold Technol, Wuhan 430074, Peoples R China. [Yang, Yuchen; Tanaka, Koichi; Liu, Jason; Anders, Andre] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Tanaka, Koichi] Mitsubishi Mat Corp, Cent Res Inst, Naka, Ibaraki 3110102, Japan. [Liu, Jason] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. RP Yang, YC (reprint author), Huazhong Univ Sci & Technol, Sch Mat Sci & Engn, State Key Lab Mat Proc & Die & Mold Technol, Wuhan 430074, Peoples R China. RI Anders, Andre/B-8580-2009; OI Anders, Andre/0000-0002-5313-6505; Tanaka, Koichi/0000-0002-3180-7881; Liu, Jason/0000-0001-9040-9253 FU China Scholarship Council; U.S. Department of Energy [DE-AC02-05CH11231] FX We gratefully acknowledge Changchun Sun of the Advanced Light Source of Berkeley Lab for providing a high speed camera. Yuchen Yang gratefully acknowledges financial support by the China Scholarship Council. Work at LBNL is supported by the U.S. Department of Energy, under Contract No. DE-AC02-05CH11231. NR 23 TC 4 Z9 4 U1 0 U2 17 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAR 23 PY 2015 VL 106 IS 12 AR 124102 DI 10.1063/1.4916233 PG 5 WC Physics, Applied SC Physics GA CE5LM UT WOS:000351876700065 ER PT J AU Yoo, HK Chang, YJ Moreschini, L Kim, HD Sohn, CH Sinn, S Oh, JS Kuo, CT Bostwick, A Rotenberg, E Noh, TW AF Yoo, Hyang Keun Chang, Young Jun Moreschini, Luca Kim, Hyeong-Do Sohn, Chang Hee Sinn, Soobin Oh, Ji Seop Kuo, Cheng-Tai Bostwick, Aaron Rotenberg, Eli Noh, Tae Won TI Insulating-layer formation of metallic LaNiO3 on Nb-doped SrTiO3 substrate SO APPLIED PHYSICS LETTERS LA English DT Article ID TRANSITIONS; SUPERLATTICES; DEVICE; FILMS; GAP AB We investigated the electronic structures of strongly correlated metallic LaNiO3 (LNO) and semiconducting Nb-doped SrTiO3 (Nb:STO) heterostructures by varying the LNO film thickness using in situ photoemission spectroscopy. We found that, contrary to other interfaces with SrTiO3 and LaAlO3, insulating LNO layers are formed between metallic LNO layers and Nb:STO. Such behavior seems to be related with an electron transfer from Nb:STO to LNO due to Schottky-barrier formation at the interface. (C) 2015 AIP Publishing LLC. C1 [Yoo, Hyang Keun; Kim, Hyeong-Do; Sohn, Chang Hee; Sinn, Soobin; Oh, Ji Seop; Kuo, Cheng-Tai; Noh, Tae Won] Inst for Basic Sci Korea, Ctr Correlated Electron Syst, Seoul 151747, South Korea. [Yoo, Hyang Keun; Kim, Hyeong-Do; Sohn, Chang Hee; Sinn, Soobin; Oh, Ji Seop; Kuo, Cheng-Tai; Noh, Tae Won] Seoul Natl Univ, Dept Phys & Astron, Seoul 151747, South Korea. [Chang, Young Jun] Univ Seoul, Dept Phys, Seoul 130743, South Korea. [Chang, Young Jun; Moreschini, Luca; Bostwick, Aaron; Rotenberg, Eli] EO Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Kim, HD (reprint author), Inst for Basic Sci Korea, Ctr Correlated Electron Syst, Seoul 151747, South Korea. EM hdkim6612@snu.ac.kr RI Rotenberg, Eli/B-3700-2009 OI Rotenberg, Eli/0000-0002-3979-8844 FU Swiss National Science Foundation (SNSF) [PBELP2-125484]; National Research Foundation of Korea [NRF-2014R1A1A1002868]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; [IBS-R009-D1] FX The authors are grateful to S. I. Hyun, J. H. Shim, H. H. Nam, S. W. Han, S. B. Lee, and H. W. Park for helpful discussion. This work was supported by IBS-R009-D1. L. M. acknowledges support by a grant from the Swiss National Science Foundation (SNSF) (Project No. PBELP2-125484). Y.J.C. acknowledges support from National Research Foundation of Korea under Grant No. NRF-2014R1A1A1002868. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 35 TC 0 Z9 0 U1 6 U2 49 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAR 23 PY 2015 VL 106 IS 12 AR 121601 DI 10.1063/1.4916225 PG 4 WC Physics, Applied SC Physics GA CE5LM UT WOS:000351876700013 ER PT J AU Zakutayev, A Stevanovic, V Lany, S AF Zakutayev, A. Stevanovic, V. Lany, S. TI Non-equilibrium alloying controls optoelectronic properties in Cu2O thin films for photovoltaic absorber applications SO APPLIED PHYSICS LETTERS LA English DT Article ID OXIDE; SEMICONDUCTORS AB Cuprous oxide (Cu2O) has recently received much attention as a candidate material for oxide photovoltaics. However, its low absorption coefficient due to the symmetry forbidden band gap and low intrinsic p-type doping level are obstacles for further advancing the performance of Cu2O thin film solar cells. Following computational predictions on the band gap, doping, and optical properties, we report combinatorial synthesis and characterization of Cu2-2xZnxO1-ySey thin film alloys and the associated device modeling results. We show that the absorption and the conductivity can be independently controlled by Se and Zn content, thereby devising a possible route to design of more efficient oxide photovoltaics and tandem solar cells. (C) 2015 AIP Publishing LLC. C1 [Zakutayev, A.; Stevanovic, V.; Lany, S.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Stevanovic, V.] Colorado Sch Mines, Dept Phys, Golden, CO 80401 USA. RP Zakutayev, A (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM andriy.zakutayev@nrel.gov OI Zakutayev, Andriy/0000-0002-3054-5525; Lany, Stephan/0000-0002-8127-8885 FU U.S. Department of Energy, office of Energy Efficiency and Renewable Energy, as a part of a Next Generation PV II project within the SunShot initiative [DE-AC36-08GO28308] FX This work was funded by U.S. Department of Energy, office of Energy Efficiency and Renewable Energy, as a part of a Next Generation PV II project within the SunShot initiative, under Contract No. DE-AC36-08GO28308 to NREL. SEM and EDX measurements by Bobby To are gratefully acknowledged. NR 37 TC 8 Z9 8 U1 2 U2 31 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAR 23 PY 2015 VL 106 IS 12 AR 123903 DI 10.1063/1.4914974 PG 4 WC Physics, Applied SC Physics GA CE5LM UT WOS:000351876700059 ER PT J AU Grice, WP Evans, PG Lawrie, B Legre, M Lougovski, P Ray, W Williams, BP Qi, B Smith, AM AF Grice, W. P. Evans, P. G. Lawrie, B. Legre, M. Lougovski, P. Ray, W. Williams, B. P. Qi, B. Smith, A. M. TI Two-Party secret key distribution via a modified quantum secret sharing protocol SO OPTICS EXPRESS LA English DT Article ID CRYPTOGRAPHY AB We present and demonstrate a novel protocol for distributing secret keys between two and only two parties based on N-party single-qubit Quantum Secret Sharing (QSS). We demonstrate our new protocol with N = 3 parties using phase-encoded photons. We show that any two out of N parties can build a secret key based on partial information from each other and with collaboration from the remaining N - 2 parties. Our implementation allows for an accessible transition between N-party QSS and arbitrary two party QKD without modification of hardware. In addition, our approach significantly reduces the number of resources such as single photon detectors, lasers and dark fiber connections needed to implement QKD. (C) 2015 Optical Society of America C1 [Grice, W. P.; Evans, P. G.; Lawrie, B.; Lougovski, P.; Ray, W.; Qi, B.; Smith, A. M.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Legre, M.] ID Quant SA, Geneva, Switzerland. [Williams, B. P.] Univ Tennessee, Dept Phys, Knoxville, TN 37996 USA. RP Grice, WP (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. EM gricew@ornl.gov RI Lawrie, Benjamin/B-7182-2016; Qi, Bing/J-5028-2014; OI Lawrie, Benjamin/0000-0003-1431-066X; Qi, Bing/0000-0001-7723-8998; Lougovski, Pavel/0000-0002-9229-1444; Grice, Warren/0000-0003-4266-4692 FU U.S. Department of Energy under the Cybersecurity for Energy Delivery Systems(CEDS) program; U.S. Department of Energy [DE-AC05-00OR22725] FX This work is supported by the U.S. Department of Energy under the Cybersecurity for Energy Delivery Systems(CEDS) program. This manuscript has been authored by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). NR 24 TC 2 Z9 2 U1 3 U2 15 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD MAR 23 PY 2015 VL 23 IS 6 BP 7300 EP 7311 DI 10.1364/OE.23.007300 PG 12 WC Optics SC Optics GA CE3YL UT WOS:000351765900031 PM 25837073 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schofbeck, R Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Lauwers, J Luyckx, S Ochesanu, S Rougny, R De Klundert, MV Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Daci, N Heracleous, N Keaveney, J Lowette, S Maes, M Olbrechts, A Python, Q Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Caillol, C Clerbaux, B De Lentdecker, G Dobur, D Favart, L Gay, APR Grebenyuk, A 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Tomei, TRFP Gregores, EM Mercadante, PG Novaes, SF Padula, SS Aleksandrov, A Genchev, V Hadjiiska, R Iaydjiev, P Marinov, A Piperov, S Rodozov, M Stoykova, S Sultanov, G Vutova, M Dimitrov, A Glushkov, I Litov, L Pavlov, B Petkov, P Bian, JG Chen, GM Chen, HS Chen, M Cheng, T Du, R Jiang, CH Plestina, R Romeo, F Tao, J Wang, Z Asawatangtrakuldee, C Ban, Y Li, Q Liu, S Mao, Y Qian, SJ Wang, D Xu, Z Zou, W Avila, C Cabrera, A Sierra, LFC Florez, C Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Polic, D Puljak, I Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Mekterovic, D Sudic, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Bodlak, M Finger, M Finger, M Assran, Y Kamel, AE Mahmoud, MA Radi, A Kadastik, M Murumaa, M Raidal, M Tiko, A Eerola, P Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Kortelainen, MJ Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E Wendland, L Talvitie, J Tuuva, T Besancon, M Couderc, F Dejardin, M Denegri, D Fabbro, B Faure, JL Favaro, C Ferri, F Ganjour, S Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Malcles, J Rander, J Rosowsky, A Titov, M Baffioni, S Beaudette, F Busson, P Chapon, E Charlot, C Dahms, T Dalchenko, M Dobrzynski, L Filipovic, N Florent, A de Cassagnac, RG Mastrolorenzo, L Mine, P Naranjo, IN Nguyen, M Ochando, C Ortona, G Paganini, P Regnard, S Salerno, R Sauvan, JB Sirois, Y Veelken, C Yilmaz, Y Zabi, A Agram, JL Andrea, J Aubin, A Bloch, D Brom, JM Chabert, EC Collard, C Conte, E Fontaine, JC Gele, D Goerlach, U Goetzmann, C Le Bihan, AC Skovpen, K Van Hove, P Gadrat, S Beauceron, S Beaupere, N Bernet, C Boudoul, G Bouvier, E Brochet, S Montoya, CAC Chasserat, J Chierici, R Contardo, D Depasse, P El Mamouni, H Fan, J Fay, J Gascon, S Gouzevitch, M Ille, B Kurca, T Lethuillier, M Mirabito, L Perries, S Alvarez, JDR Sabes, D Sgandurra, L Sordini, V Donckt, MV Verdier, P Viret, S Xiao, H 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A Hartmann, F Hauth, T Husemann, U Katkov, I Kornmayer, A Pardo, PL Mozer, MU Muller, T Muller, T Nurnberg, A Quast, G Rabbertz, K Rocker, S Simonis, HJ Stober, FM Ulrich, R Wagner-Kuhr, J Wayand, S Weiler, T Wolf, R Anagnostou, G Daskalakis, G Geralis, T Giakoumopoulou, VA Kyriakis, A Loukas, D Markou, A Markou, C Psallidas, A Topsis-Giotis, I Agapitos, A Kesisoglou, S Panagiotou, A Saoulidou, N Stiliaris, E Aslanoglou, X Evangelou, I Flouris, G Foudas, C Kokkas, P Manthos, N Papadopoulos, I Paradas, E Strologas, J Bencze, G Hajdu, C Hidas, P Horvath, D Sikler, F Veszpremi, V Vesztergombi, G Zsigmond, AJ Beni, N Czellar, S Karancsi, J Molnar, J Palinkas, J Szillasi, Z Makovec, A Raics, P Trocsanyi, ZL Ujvari, B Swain, SK Beri, SB Bhatnagar, V Gupta, R Bhawandeep, U Kalsi, AK Kaur, M Kumar, R Mittal, M Nishu, N Singh, JB Kumar, A Kumar, A Ahuja, S Bhardwaj, A Choudhary, BC Kumar, A Malhotra, S Naimuddin, M Ranjan, K Sharma, V Banerjee, S Bhattacharya, S Chatterjee, K Dutta, S Gomber, B 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Smith, W. H. Taylor, D. Vuosalo, C. Woods, N. CA CMS Collaboration TI Search for supersymmetry using razor variables in events with b-tagged jets in pp collisions at root s=8 TeV SO PHYSICAL REVIEW D LA English DT Article ID FINE-TUNING PROBLEM; SQUARK; EXTENSION; NEUTRINO; BREAKING; MODELS; BOSON; LHC AB An inclusive search for supersymmetry in events with at least one b-tagged jet is performed using proton-proton collision data collected by the CMS experiment in 2012 at a center-of-mass energy of 8 TeV. The data set size corresponds to an integrated luminosity of 19.3 fb(-1). The two-dimensional distribution of the razor variables R-2 and M-R is studied in events with and without leptons. The data are found to be consistent with the expected background, which is modeled with an empirical function. Exclusion limits on supersymmetric particle masses at a 95% confidence level are derived in several simplified supersymmetric scenarios for several choices of the branching fractions. By combining the likelihoods of a search in events without leptons and a search that requires a single lepton (electron or muon), an improved bound on the top-squark mass is obtained. Assuming the lightest supersymmetric particle to be stable and weakly interacting, and to have a mass of 100 GeV, the branching-fraction-dependent (-independent) production of gluinos is excluded for gluino masses up to 1310 (1175) GeV. The corresponding limit for top-squark pair production is 730 (645) GeV. C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Bergauer, T.; Dragicevic, M.; Eroe, J.; Friedl, M.; Fruehwirth, R.; Ghete, V. M.; Hartl, C.; Hoermann, N.; Hrubec, J.; Jeitler, M.; Kiesenhofer, W.; Knuenz, V.; Krammer, M.; Kraetschmer, I.; Liko, D.; Mikulec, I.; Rabady, D.; Rahbaran, B.; Rohringer, H.; Schoefbeck, R.; Strauss, J.; Treberer-Treberspurg, W.; Waltenberger, W.; Wulz, C. -E.] OeAW, Inst Hochenergiephys, Vienna, Austria. 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E.; Fiorendi, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Manzoni, R. A.; Martelli, A.; Marzocchi, B.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Di Guida, S.; Fabozzi, F.; Iorio, A. O. M.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Iorio, A. O. M.] Univ Naples Federico II, Naples, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata Potenza, Naples, Italy. [Di Guida, S.; Meola, S.] Univ G Marconi Roma, Naples, Italy. [Azzi, P.; Bacchetta, N.; Bisello, D.; Branca, A.; Carlin, R.; Checchia, P.; Dall'Osso, M.; Dorigo, T.; Dosselli, U.; Galanti, M.; Gasparini, U.; Gonella, F.; Gozzelino, A.; Gulmini, M.; Kanishchev, K.; Lacaprara, S.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Zotto, P.; Zucchetta, A.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Bisello, D.; Branca, A.; Carlin, R.; Dall'Osso, M.; Galanti, M.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.] Univ Padua, Padua, Italy. [Kanishchev, K.] Univ Trento Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Biasini, M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. 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[Barone, L.; D'imperio, G.; Del Re, D.; Longo, E.; Margaroli, F.; Micheli, F.; Organtini, G.; Rahatlou, S.; Santanastasio, F.; Soffi, L.; Traczyk, P.; Colafranceschi, S.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Degano, A.; Demaria, N.; Finco, L.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Casasso, S.; Costa, M.; Degano, A.; Finco, L.; Migliore, E.; Monaco, V.; Pacher, L.; Angioni, G. L. Pinna; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Schizzi, A.; Umer, T.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Schizzi, A.; Umer, T.; Zanetti, A.] Univ Trieste, Trieste, Italy. [Chang, S.; Kropivnitskaya, A.; Nam, S. K.] Kangweon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Park, H.; Sakharov, A.; Son, D. C.; Kamon, T.] Kyungpook Natl Univ, Daegu, South Korea. [Kim, T. J.; Ryu, M. S.] Chonbuk Natl Univ, Jeonju 561756, South Korea. [Kim, J. Y.; Moon, D. H.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, Y.; Lee, B.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Yoo, H. D.] Seoul Natl Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, I. C.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, D.; Kwon, E.; Lee, J.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.] Vilnius Univ, Vilnius, Lithuania. [Komaragiri, J. R.; Ali, M. A. B. Md] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Casimiro Linares, E.; Castilla-Valdez, H.; De la Cruz-Burelo, E.; Heredia-de la Cruz, I.; Hernandez-Almada, A.; Lopez-Fernandez, R.; Sanchez-Hernandez, A.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Montoya, C. A. Carrillo; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Pedraza, I.; Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Reucroft, S.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, A.; Ahmad, M.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz E Silva, C.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Lloret Iglesias, L.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Tsamalaidze, Z.; Abdulsalam, A.; Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.; Smirnov, I.; Adair, A.] Joint Inst Nucl Res, Dubna, Russia. [Smirnov, V.; Golovtsov, V.; Ivanov, Y.; Kim, V.; Kuznetsova, E.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Matveev, V.; Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Pozdnyakov, I.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Popov, A.; Zhukov, V.; Katkov, I.; Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Fed, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.; Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.; Milenovic, P.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia. [Alcaraz Maestre, J.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De la Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Graziano, A.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Rabady, D.; Pernie, L.; Genchev, V.; Boudoul, G.; Contardo, D.; Lingemann, J.; Hartmann, F.; Kornmayer, A.; Mohanty, A. K.; Radogna, R.; Sharma, A.; Silvestris, L.; Giordano, F.; Gennai, S.; Gerosa, R.; Lucchini, M. T.; Marzocchi, B.; Di Guida, S.; Meola, S.; Paolucci, P.; Ciangottini, D.; Spiezia, A.; Donato, S.; Palla, F.; Micheli, F.; Traczyk, P.; Casasso, S.; Finco, L.; Candelise, V.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; David, A.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dorney, B.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Franzoni, G.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Hansen, M.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Magini, N.; Malgeri, L.; Mannelli, M.; Marrouche, J.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Orsini, L.; Pape, L.; Perez, E.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Pimiae, M.; Piparo, D.; Plagge, M.; Racz, A.; Rolandi, G.; Rovere, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Steggemann, J.; Stieger, B.; Stoye, M.; Takahashi, Y.; Treille, D.; Tsirou, A.; Veres, G. 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Millan; Ngadiuba, J.; Pinna, D.; Robmann, P.; Ronga, F. J.; Taroni, S.; Verzetti, M.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Chang, P.; Chang, Y. H.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Grundler, U.; Hou, W. -S.; Liu, Y. F.; Lu, R. -S.; Petrako, E.; Tzeng, Y. M.; Wilken, R.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Fac Sci, Dept Phys, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Gamsizkan, H.; Isildak, B.; Karapinar, G.; Ocalan, K.; Sekmen, S.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Albayrak, E. A.; Gulmez, E.; Kaya, M.; Kaya, O.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cankocak, K.; Vardarli, F. I.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Kharkov Phys & Technol Inst, Natl Sci Ctr, UA-310108 Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Sakuma, T.; El Nasr-Storey, S. Seif; Senkin, S.; Smith, V. J.] Univ Bristol, Bristol, Avon, England. [Belyaev, A.; Newbold, D. M.; Bell, K. W.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Williams, T.; Womersley, W. J.; Worm, S. D.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Dauncey, P.; Davies, G.; Negra, M. Della; Dunne, P.; Ferguson, W.; Fulcher, J.; Futyan, D.; Hall, G.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Mathias, B.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.; Wu, Z.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Lawson, P.; Richardson, C.; Rohlf, J.; St John, J.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Bhattacharya, S.; Alimena, J.; Berry, E.; Christopher, G.; Cutts, D.; Demiragli, Z.; Dhingra, N.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.; Swanson, J.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De la Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Lander, R.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. 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Trocsanyi, Zoltan/0000-0002-2129-1279 FU Science and Technology Facilities Council [CMS, ST/K001604/1] NR 74 TC 10 Z9 10 U1 8 U2 46 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 23 PY 2015 VL 91 IS 5 AR 052018 DI 10.1103/PhysRevD.91.052018 PG 28 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CE1LL UT WOS:000351573100001 ER PT J AU Zhong, ZC Si, L Zhang, QF Yin, WG Yunoki, S Held, K AF Zhong, Zhicheng Si, Liang Zhang, Qinfang Yin, Wei-Guo Yunoki, Seiji Held, Karsten TI Giant Switchable Rashba Effect in Oxide Heterostructures SO ADVANCED MATERIALS INTERFACES LA English DT Article DE oxide heterostructures; spin orbit coupling; rashba effect; ferroelectricity ID LOCALIZED WANNIER FUNCTIONS; SPIN; PLANE; FERROELECTRICITY; PRESSURE; DYNAMICS; BITEI; FILMS AB One of the most fundamental phenomena and a reminder of the electron's relativistic nature is the Rashba spin splitting for broken inversion symmetries in two-dimensional condensed matter systems. Typically, this splitting is a tiny relativistic correction. By coupling ferroelectric BaTiO3 and a 5d (or 4d) transition metal oxide with a large spin-orbit coupling, Ba(Os,Ir,Ru)O-3, it is shown that giant Rashba spin splittings are indeed possible and even controllable by an external electric field. Based on density functional theory and a microscopic tight binding understanding, it is concluded that the electric field is amplified and stored as a ferroelectric Ti-O distortion which, through the network of oxygen octahedra, induces a large (Os,Ir,Ru)-O distortion. The BaTiO3/Ba(Os,Ru,Ir)O-3 heterostructure is hence the ideal test station for switching and studying the Rashba effect and allows applications at room temperature. C1 [Zhong, Zhicheng; Si, Liang; Held, Karsten] Vienna Univ Technol, Inst Solid State Phys, A-1040 Vienna, Austria. [Zhang, Qinfang] Yancheng Inst Technol, Key Lab Adv Technol Environm Protect Jiangsu Prov, Yancheng, Peoples R China. [Yin, Wei-Guo] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Yunoki, Seiji] RIKEN, Computat Condensed Matter Phys Lab, Wako, Saitama 35110198, Japan. [Yunoki, Seiji] RIKEN, Computat Mat Sci Res Team, Adv Inst Computat Sci, Kobe, Hyogo 6500047, Japan. [Yunoki, Seiji] RIKEN, Computat Quantum Matter Res Team, Ctr Emergent Matter Sci, Wako, Saitama 3510198, Japan. RP Zhong, ZC (reprint author), Vienna Univ Technol, Inst Solid State Phys, A-1040 Vienna, Austria. EM Zhicheng.Zhong@ifp.tuwien.ac.at RI Zhang, Qinfang/C-6481-2008; Yunoki, Seiji/B-1831-2008; Zhong, Zhicheng/B-7675-2009; Held, Karsten/O-4178-2015; Yin, Weiguo/A-9671-2014 OI Zhang, Qinfang/0000-0003-3233-3400; Zhong, Zhicheng/0000-0003-1507-4814; Held, Karsten/0000-0001-5984-8549; Yin, Weiguo/0000-0002-4965-5329 FU Austrian Science Fund through the SFB [Vi-CoM F4103-N13]; NSFC [11474246, 11204265]; NSF of Jiangsu Province [BK2012248]; U.S. Department of Energy [DE-AC02-98CH10886]; MEXT Japan [25287096]; RIKEN iTHES Project; European Research Council under the European Union [306447] FX Z.Z. acknowledges financial support by the Austrian Science Fund through the SFB Vi-CoM F4103-N13, Q.F.Z by NSFC (11474246, 11204265), the NSF of Jiangsu Province (BK2012248), W.Y. by the U.S. Department of Energy under Contract No. DE-AC02-98CH10886, S.Y. by Grant-in-Aid for Science Research from MEXT Japan under the grant number 25287096 and by RIKEN iTHES Project, and KH by the European Research Council under the European Union's Seventh Framework Program (FP/2007-2013)/ERC through grant agreement n. 306447. Calculations have been done on the Vienna Scientific Cluster (VSC). NR 44 TC 0 Z9 0 U1 4 U2 54 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 2196-7350 J9 ADV MATER INTERFACES JI Adv. Mater. Interfaces PD MAR 23 PY 2015 VL 2 IS 5 DI 10.1002/admi.201400445 PG 5 WC Chemistry, Multidisciplinary; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CE2FD UT WOS:000351628800008 ER PT J AU Carrasco, J Lopez-Duran, D Liu, ZY Duchon, T Evans, J Senanayake, SD Crumlin, EJ Matolin, V Rodriguez, JA Ganduglia-Pirovano, MV AF Carrasco, Javier Lopez-Duran, David Liu, Zongyuan Duchon, Tomas Evans, Jaime Senanayake, Sanjaya D. Crumlin, Ethan J. Matolin, Vladimir Rodriguez, Jose A. Veronica Ganduglia-Pirovano, M. TI In Situ and Theoretical Studies for the Dissociation of Water on an Active Ni/CeO2 Catalyst: Importance of Strong Metal-Support Interactions for the Cleavage of O-H Bonds SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE ceria; density functional calculations; nickel; water dissociation; X-ray photoelectron spectroscopy ID GAS SHIFT REACTION; FUNDAMENTAL-ASPECTS; CEO2(111) SURFACE; SOLID-SURFACES; ADSORPTION; MECHANISM; NI(111); AU; CE1-XNIXO2-Y; PLATINUM AB Water dissociation is crucial in many catalytic reactions on oxide-supported transition-metal catalysts. Supported by experimental and density-functional theory results, the effect of the support on O-H bond cleavage activity is elucidated for nickel/ceria systems. Ambient-pressure O1s photoemission spectra at low Ni loadings on CeO2(111) reveal a substantially larger amount of OH groups as compared to the bare support. Computed activation energy barriers for water dissociation show an enhanced reactivity of Ni adatoms on CeO2(111) compared with pyramidal Ni-4 particles with one Ni atom not in contact with the support, and extended Ni(111) surfaces. At the origin of this support effect is the ability of ceria to stabilize oxidized Ni2+ species by accommodating electrons in localized f-states. The fast dissociation of water on Ni/CeO2 has a dramatic effect on the activity and stability of this system as a catalyst for the water-gas shift and ethanol steam reforming reactions. C1 [Carrasco, Javier; Lopez-Duran, David; Veronica Ganduglia-Pirovano, M.] CSIC, Inst Catalisis & Petroleoquim, Madrid 28049, Spain. [Liu, Zongyuan; Senanayake, Sanjaya D.; Rodriguez, Jose A.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Duchon, Tomas; Matolin, Vladimir] Charles Univ Prague, Fac Math & Phys, Prague 8, Czech Republic. [Evans, Jaime] Cent Univ Venezuela, Fac Ciencias, Caracas 1020A, Venezuela. [Crumlin, Ethan J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Carrasco, Javier; Lopez-Duran, David] CIC Energigune, Minano 01510, Alava, Spain. [Liu, Zongyuan; Rodriguez, Jose A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11749 USA. RP Carrasco, J (reprint author), CSIC, Inst Catalisis & Petroleoquim, C Marie Curie 2, Madrid 28049, Spain. EM rodrigez@bnl.gov; vgp@icp.csic.es RI Carrasco, Javier/I-5488-2015; COST, CM1104/I-8057-2015; Senanayake, Sanjaya/D-4769-2009 OI Carrasco, Javier/0000-0003-3117-6933; Senanayake, Sanjaya/0000-0003-3991-4232 FU MINECO-Spain [CTQ2012-32928]; Ministry of Education of the Czech Republic [LH11017]; U.S. Department of Energy [DE-AC02-98CH10886, DE-AC02-05CH11231]; Ramon y Cajal Fellowship; Marie Curie Career Integration Grant FP7-PEOPLE-CIG: Project NanoWGS; Royal Society through the Newton Alumnus scheme FX This work has been supported by the MINECO-Spain (CTQ2012-32928), the Ministry of Education of the Czech Republic (LH11017), and the U.S. Department of Energy (DE-AC02-98CH10886, DE-AC02-05CH11231). J.C. acknowledges support by the Ramon y Cajal Fellowship, the Marie Curie Career Integration Grant FP7-PEOPLE-2011-CIG: Project NanoWGS and The Royal Society through the Newton Alumnus scheme. The COST action CM1104 is gratefully acknowledged. Computer time provided by the SGAI-CSIC, CESGA, BIFI-ZCAM, IFCA, and the BSC is acknowledged. NR 36 TC 38 Z9 38 U1 40 U2 204 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD MAR 23 PY 2015 VL 54 IS 13 BP 3917 EP 3921 DI 10.1002/anie.201410697 PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA CD6NA UT WOS:000351204600009 PM 25651288 ER PT J AU Luo, X Stanev, V Shen, B Fang, L Ling, XS Osborn, R Rosenkranz, S Benseman, TM Divan, R Kwok, WK Welp, U AF Luo, X. Stanev, V. Shen, B. Fang, L. Ling, X. S. Osborn, R. Rosenkranz, S. Benseman, T. M. Divan, R. Kwok, W. -K. Welp, U. TI Antiferromagnetic and nematic phase transitions in BaFe2(As1=xPx)(2) studied by ac microcalorimetry and SQUID magnetometry SO PHYSICAL REVIEW B LA English DT Article ID HIGH-TEMPERATURE SUPERCONDUCTIVITY; IRON ARSENIDE SUPERCONDUCTOR; MAGNETIC-SUSCEPTIBILITY; DETWINNED BA(FE1-XCOX)(2)AS-2; ORDER; LAO1-XFXFEAS; ANISOTROPY; PNICTIDES; SYSTEMS; STATES AB We study the antiferromagnetic (AFM) and structural phase transitions in single-crystal BaFe2(As-1-(x) P-x)(2) (x = 0, 0.3) at temperatures TN and TS, respectively, by high-resolution ac microcalorimetry and SQUID magnetometry. The specific heat measurements of both as-grown and annealed BaFe2As2 display a sharp peak at the AFMs-tructural transitions. A kink in the entropy of annealed BaFe2As2 gives evidence for splitting of the two transitions by approximately 0.5 K. No additional features could be identified in the specific heat of both BaFe2As2 and BaFe2(As0.7P0.3)(2) in the temperature regions around T* > TS where torque measurements [S. Kasahara et al., Nature 486, 382 (2012)] had revealed the "true" nematic phase transition, even though the Ginzburg-Landau model used to fit the magnetic torque data indicates that the expected thermal anomaly should be easily observable with our experimental resolution. C1 [Luo, X.; Stanev, V.; Shen, B.; Fang, L.; Osborn, R.; Rosenkranz, S.; Benseman, T. M.; Kwok, W. -K.; Welp, U.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Luo, X.; Ling, X. S.] Brown Univ, Dept Phys, Providence, RI 02912 USA. [Stanev, V.] Univ Maryland, Dept Phys, College Pk, MD 20742 USA. [Benseman, T. M.] Univ Illinois, Dept Phys, Chicago, IL 60607 USA. [Divan, R.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. RP Luo, X (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM xluo@anl.gov; welp@anl.gov RI Rosenkranz, Stephan/E-4672-2011; Shen, Bing/G-6514-2016 OI Rosenkranz, Stephan/0000-0002-5659-0383; FU US Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; Center for Emergent Superconductivity, an Energy Frontier Research Center - US Department of Energy, Office of Science, Office of Basic Energy Sciences FX We would like to thank R. M. Fernandes, F. Hardy, and A. E. B ohmer for fruitful discussions. This work was primarily supported by the US Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. Use of the Center for Nanoscale Materials was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. Crystal synthesis was supported by the Center for Emergent Superconductivity, an Energy Frontier Research Center funded by the US Department of Energy, Office of Science, Office of Basic Energy Sciences. NR 53 TC 4 Z9 4 U1 5 U2 31 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAR 23 PY 2015 VL 91 IS 9 AR 094512 DI 10.1103/PhysRevB.91.094512 PG 6 WC Physics, Condensed Matter SC Physics GA CE0QB UT WOS:000351508400004 ER PT J AU Velizhanin, KA AF Velizhanin, Kirill A. TI Geometric universality of plasmon modes in graphene nanoribbon arrays SO PHYSICAL REVIEW B LA English DT Article ID TERAHERTZ; NANOSTRUCTURES AB Graphene plasmonics is a rapidly growing field with multiple potential applications. One of the standard ways to study plasmons in graphene is by fabricating an array of graphene nanoribbons where nanoribbon edges provide the efficient photon-plasmon coupling. We systematically analyze the problem of optical plasmonic response in such systems and demonstrate the purely geometric nature of the size quantization condition for graphene plasmons. Accurate numerical calculations allowed us to tabulate the universal geometric parameters of plasmon size quantization, which is expected to become useful in analysis of experimental data on plasmonic response of graphene nanoribbons. A simple analytical theory has also been developed, which accurately reproduces all the qualitative features of optical plasmonic response of graphene nanoribbons. C1 Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Velizhanin, KA (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM kirill@lanl.gov RI Velizhanin, Kirill/C-4835-2008 FU NNSA of the U.S. DOE at LANL FX We are thankful to Anatoly Efimov for multiple discussions and the help with the manuscript. This work was performed under the NNSA of the U.S. DOE at LANL under Contract No. DE-AC52-06NA25396. NR 30 TC 3 Z9 3 U1 4 U2 23 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAR 23 PY 2015 VL 91 IS 12 AR 125429 DI 10.1103/PhysRevB.91.125429 PG 7 WC Physics, Condensed Matter SC Physics GA CE0QM UT WOS:000351509500005 ER PT J AU Wang, LW AF Wang, Lin-Wang TI Fully self-consistent solution of the Dyson equation using a plane-wave basis set SO PHYSICAL REVIEW B LA English DT Article ID QUASI-PARTICLE CALCULATIONS; GW APPROXIMATION; SEMICONDUCTORS; SOLIDS; CONSERVATION; ENERGIES; STATES AB Self-consistent solutions of the Dyson equation are obtained using a plane-wave basis set for seven small molecules. Such self-consistent solutions can help to unify the different GW self-consistent schemes, reduce the scatter of results in current GW calculations, and shed light on the true effects of GW self-consistency. Unlike other works of self-consistent GW calculations, in the present work the Green's function is expressed as a matrix under the plane-wave basis set. The algorithmic details which enable such calculations are presented. The ability to solve the full Green's function using a plane-wave basis set may open the door for future beyond-GW many-body perturbation theory calculations. C1 Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Wang, LW (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. FU Office of Science (SC), Basic Energy Science (BES), Materials Science and Engineering Division (MSED), of the US Department of Energy (DOE) [DE-AC02-05CH11231] FX We like to thank Prof. Rex Godby for helpful discussions. This work was supported by the Director, Office of Science (SC), Basic Energy Science (BES), Materials Science and Engineering Division (MSED), of the US Department of Energy (DOE) under Contract No. DE-AC02-05CH11231 through the Materials Theory program. It used resources of the National Energy Research Scientific Computing Center (NERSC) and Oak Ridge Leadership Computing Facility (OLCF) with the computational time allocated by the Innovative and Novel Computational Impact on Theory and Experiment (INCITE) project. NR 47 TC 5 Z9 5 U1 1 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAR 23 PY 2015 VL 91 IS 12 AR 125135 DI 10.1103/PhysRevB.91.125135 PG 9 WC Physics, Condensed Matter SC Physics GA CE0QM UT WOS:000351509500003 ER PT J AU Weisberg, A Aceves, SM AF Weisberg, Andrew Aceves, Salvador M. TI The potential of dry winding for rapid, inexpensive manufacture of composite overwrapped pressure vessels SO INTERNATIONAL JOURNAL OF HYDROGEN ENERGY LA Russian DT Article DE Pressure vessel manufacture; Rapid winding ID HYDROGEN STORAGE AB We are proposing a methodology for reducing manufacturing time and cost of composite overwrapped pressure vessels (COPVs). Dry winding methodology promises to increase bonding speed enabling rapid vessel winding (10 min vs. 3 h with today's wet winding approach) with no need for oven curing. Faster winding is likely to reduce vessel cost due to higher throughput enabling increased productivity from expensive winding machines as well as reduced labor cost per vessel. Tape manufacture in large scale in a central facility minimizes tape handling and distribution costs. Finally, high ratio of fiber to resin reduces resin cost as well as the wall thickness for any necessary strength, increasing the packaging efficiency of the vessel and reducing weight. Copyright (C) 2015, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved. C1 [Weisberg, Andrew; Aceves, Salvador M.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RP Aceves, SM (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave,L-792, Livermore, CA 94551 USA. EM saceves@llnl.gov FU DOE, Office of Fuel Cell Technologies, Jesse Adams, Technology Development Manager; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This project was funded by DOE, Office of Fuel Cell Technologies, Jesse Adams, Technology Development Manager. This work performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 8 TC 0 Z9 0 U1 3 U2 3 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-3199 EI 1879-3487 J9 INT J HYDROGEN ENERG JI Int. J. Hydrog. Energy PD MAR 22 PY 2015 VL 40 IS 11 BP 4207 EP 4211 DI 10.1016/j.ijhydene.2015.01.130 PG 5 WC Chemistry, Physical; Electrochemistry; Energy & Fuels SC Chemistry; Electrochemistry; Energy & Fuels GA CF7PT UT WOS:000352749500019 ER PT J AU Chelikowsky, JR Cohen, ML AF Chelikowsky, James R. Cohen, Marvin L. TI Semiconductors: A pillar of pure and applied physics SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID NORM-CONSERVING PSEUDOPOTENTIALS; BORON-NITRIDE NANOTUBES; WAVE-FUNCTIONS; TOTAL-ENERGY; SUPERCONDUCTIVITY; SI; GE; SILICON; SOLIDS AB We give an overview of the central role semiconductor research that has played in basic, applied, and computational science. Our focus is on basic science. However, we will make general comments about applications, such as the transistor, integrated circuits, solar devices, and lasers, which evolved from basic research, and about simulations using computational science, which has enormously benefited from semiconductor research. We will make reference to links with other branches of physics and more generally other areas of science and fields like electrical engineering, computer science, material science, medical science, and chemistry that have made significant contributions to our everyday life. (C) 2015 AIP Publishing LLC. C1 [Chelikowsky, James R.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Chelikowsky, James R.] Univ Texas Austin, Dept Chem Engn, Austin, TX 78712 USA. [Chelikowsky, James R.] Univ Texas Austin, Ctr Computat Mat, Inst Computat Engn & Sci, Austin, TX 78712 USA. [Cohen, Marvin L.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Cohen, Marvin L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Chelikowsky, JR (reprint author), Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. FU NSF [DMR-10-1006184]; theory program at the Lawrence Berkeley National Laboratory through the Office of Basic Science, U.S. Department of Energy [DE-AC02-05CH11231]; Department of Energy by the Scientific Discovery through Advanced Computing (SciDAC) program - U.S. Department of Energy, Office of Science, Advanced Scientific Computing Research and Basic Energy Sciences [DE-FG02-06ER46286, DESC0008877] FX M.L.C. wishes to acknowledge support from NSF Grant No. DMR-10-1006184 and the theory program at the Lawrence Berkeley National Laboratory through the Office of Basic Science, U.S. Department of Energy under Contract No. DE-AC02-05CH11231. J.R.C. wishes acknowledge support from the Department of Energy for work on nanostructures from Grant No. DE-FG02-06ER46286 support provided by the Scientific Discovery through Advanced Computing (SciDAC) program funded by U.S. Department of Energy, Office of Science, Advanced Scientific Computing Research and Basic Energy Sciences under Award No. DESC0008877 on algorithms. NR 35 TC 2 Z9 2 U1 1 U2 14 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAR 21 PY 2015 VL 117 IS 11 AR 112812 DI 10.1063/1.4913838 PG 8 WC Physics, Applied SC Physics GA CE1WZ UT WOS:000351604900013 ER PT J AU McCluskey, MD Corolewski, CD Lv, JP Tarun, MC Teklemichael, ST Walter, ED Norton, MG Harrison, KW Ha, S AF McCluskey, Matthew D. Corolewski, Caleb D. Lv, Jinpeng Tarun, Marianne C. Teklemichael, Samuel T. Walter, Eric D. Norton, M. Grant Harrison, Kale W. Ha, Su TI Acceptors in ZnO SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID ZINC-OXIDE; COPPER IMPURITIES; LUMINESCENCE; NANOCRYSTALS; EMISSION; CRYSTALS; CLUSTERS; SURFACE; CU; SEMICONDUCTORS AB Zinc oxide (ZnO) has potential for a range of applications in the area of optoelectronics. The quest for p-type ZnO has focused much attention on acceptors. In this paper, Cu, N, and Li acceptor impurities are discussed. Experimental evidence indicates these point defects have acceptor levels 3.2, 1.4, and 0.8 eV above the valence-band maximum, respectively. The levels are deep because the ZnO valence band is quite low compared to conventional, non-oxide semiconductors. Using MoO2 contacts, the electrical resistivity of ZnO:Li was measured and showed behavior consistent with bulk hole conduction for temperatures above 400 K. A photoluminescence peak in ZnO nanocrystals is attributed to an acceptor, which may involve a Zn vacancy. High field (W-band) electron paramagnetic resonance measurements on the nanocrystals revealed an axial center with g(perpendicular to) = 2.0015 and g(//) = 2.0056, along with an isotropic center at g = 2.0035. (C) 2015 AIP Publishing LLC. C1 [McCluskey, Matthew D.; Corolewski, Caleb D.; Lv, Jinpeng; Tarun, Marianne C.; Teklemichael, Samuel T.] Washington State Univ, Dept Phys & Astron, Pullman, WA 99164 USA. [Walter, Eric D.] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Norton, M. Grant; Harrison, Kale W.] Washington State Univ, Sch Mech & Mat Engn, Pullman, WA 99164 USA. [Ha, Su] Washington State Univ, Voiland Sch Chem Engn & Bioengn, Pullman, WA 99164 USA. RP McCluskey, MD (reprint author), Washington State Univ, Dept Phys & Astron, Pullman, WA 99164 USA. EM mattmcc@wsu.edu RI Walter, Eric/P-9329-2016; OI McCluskey, Matthew/0000-0002-0786-4106 FU Department of Energy (DOE) [DE-FG02-07ER46386]; National Science Foundation (NSF) [DMR-1202532, CBET-1034308]; DOE's Office of Biological and Environmental Research; Office of Naval Research [N00014-12-1-0830] FX This work was supported by Department of Energy (DOE) Grant No. DE-FG02-07ER46386, with partial student support (CDC) provided by National Science Foundation (NSF) Grant No. DMR-1202532. EPR measurements (EDW, STT) were performed using EMSL, a national scientific user facility sponsored by the DOE's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. MoO2 research (MGN, KWH, SH) was supported by NSF Grant No. CBET-1034308 and the Office of Naval Research (N00014-12-1-0830). NR 69 TC 12 Z9 12 U1 6 U2 59 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAR 21 PY 2015 VL 117 IS 11 AR 112802 DI 10.1063/1.4913827 PG 6 WC Physics, Applied SC Physics GA CE1WZ UT WOS:000351604900003 ER PT J AU Pilania, G Uberuaga, BP AF Pilania, G. Uberuaga, B. P. TI Cation ordering and effect of biaxial strain in double perovskite CsRbCaZnCl6 SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID FUNCTIONAL PERTURBATION-THEORY; FERROELECTRIC THIN-FILMS; B-SITE ORDER; A-SITE; FUEL-CELLS; OXIDES; CRYSTAL; POLARIZATION; CATALYSTS; BOUNDARY AB Here, we investigate the electronic structure, energetics of cation ordering, and effect of biaxial strain on double perovskite CsRbCaZnCl6 using first-principles calculations based on density functional theory. The two constituents (i.e., CsCaCl3 and RbZnCl3) forming the double perovskite exhibit a stark contrast. While CsCaCl3 is known to exist in a cubic perovskite structure and does not show any epitaxial strain induced phase transitions within an experimentally accessible range of compressive strains, RbZnCl3 is thermodynamically unstable in the perovskite phase and exhibits ultra-sensitive response at small epitaxial strains if constrained in the perovskite phase. We show that combining the two compositions in a double perovskite structure not only improves overall stability but also the strain-polarization coupling of the material. Our calculations predict a ground state with P4/nmm space group for the double perovskite, where A-site cations (i.e., Cs and Rb) are layer-ordered and B-site cations (i.e., Ca and Zn) prefer a rocksalt type ordering. The electronic structure and bandgap in this system are shown to be quite sensitive to the B-site cation ordering and is minimally affected by the ordering of A-site cations. We find that at experimentally accessible compressive strains CsRbCaZnCl6 can be phase transformed from its paraelectric ground state to an antiferroelectric state, where Zn atoms contribute predominantly to the polarization. Furthermore, both energy difference and activation barrier for a transformation between this antiferroelectric state and the corresponding ferroelectric configuration are predicted to be small. The computational approach presented here opens a new pathway towards a rational design of novel double perovskites with improved strain response and functionalities. (C) 2015 AIP Publishing LLC. C1 [Pilania, G.; Uberuaga, B. P.] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. RP Pilania, G (reprint author), Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. EM gpilania@lanl.gov RI Albe, Karsten/F-1139-2011; OI Pilania, Ghanshyam/0000-0003-4460-1572 FU U.S. Department of Energy through the LANL/LDRD Program; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; National Nuclear Security Administration of the (U.S.) Department of Energy [DE-AC52-06NA25396] FX G.P. gratefully acknowledges the support of the U.S. Department of Energy through the LANL/LDRD Program for this work. B.P.U. would like to acknowledge support by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. Los Alamos National Laboratory is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the (U.S.) Department of Energy under Contract No. DE-AC52-06NA25396. NR 78 TC 3 Z9 3 U1 3 U2 23 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAR 21 PY 2015 VL 117 IS 11 AR 114103 DI 10.1063/1.4915938 PG 9 WC Physics, Applied SC Physics GA CE1WZ UT WOS:000351604900033 ER PT J AU Upadhyay, J Im, D Popovic, S Valente-Feliciano, AM Phillips, L Vuskovic, L AF Upadhyay, J. Im, Do Popovic, S. Valente-Feliciano, A. -M. Phillips, L. Vuskovic, L. TI Etching mechanism of niobium in coaxial Ar/Cl-2 radio frequency plasma SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID TEMPERATURE-DEPENDENCE; GLOW-DISCHARGES; ION; ETCHER; GAAS AB The understanding of the Ar/Cl-2 plasma etching mechanism is crucial for the desired modification of inner surface of the three dimensional niobium (Nb) superconductive radio frequency cavities. Uniform mass removal in cylindrical shaped structures is a challenging task because the etch rate varies along the direction of gas flow. The study is performed in the asymmetric coaxial radio-frequency (rf) discharge with two identical Nb rings acting as a part of the outer electrode. The dependence of etch rate uniformity on pressure, rf power, dc bias, Cl-2 concentration, diameter of the inner electrode, temperature of the outer cylinder, and position of the samples in the structure is determined. To understand the plasma etching mechanisms, we have studied several factors that have important influence on the etch rate and uniformity, which include the plasma sheath potential, Nb surface temperature, and the gas flow rate. (C) 2015 AIP Publishing LLC. C1 [Upadhyay, J.; Im, Do; Popovic, S.; Vuskovic, L.] Old Dominion Univ, Dept Phys, Ctr Accelerator Sci, Norfolk, VA 23529 USA. [Valente-Feliciano, A. -M.; Phillips, L.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. RP Upadhyay, J (reprint author), Old Dominion Univ, Dept Phys, Ctr Accelerator Sci, Norfolk, VA 23529 USA. FU Office of High Energy Physics, Office of Science, Department of Energy [DE-SC0007879]; Thomas Jefferson National Accelerator Facility, Accelerator Division through JSA/DOE [DE-AC05-06OR23177] FX This work was supported by the Office of High Energy Physics, Office of Science, Department of Energy under Grant No. DE-SC0007879. Thomas Jefferson National Accelerator Facility, Accelerator Division supports J. Upadhyay through fellowship under JSA/DOE Contract No. DE-AC05-06OR23177. NR 20 TC 2 Z9 2 U1 1 U2 8 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAR 21 PY 2015 VL 117 IS 11 AR 113301 DI 10.1063/1.4914298 PG 7 WC Physics, Applied SC Physics GA CE1WZ UT WOS:000351604900023 ER PT J AU Yan, YF Yin, WJ Wu, YL Shi, TT Paudel, NR Li, C Poplawsky, J Wang, ZW Moseley, J Guthrey, H Moutinho, H Pennycook, SJ Al-Jassim, MM AF Yan, Yanfa Yin, Wan-Jian Wu, Yelong Shi, Tingting Paudel, Naba R. Li, Chen Poplawsky, Jonathan Wang, Zhiwei Moseley, John Guthrey, Harvey Moutinho, Helio Pennycook, Stephen J. Al-Jassim, Mowafak M. TI Physics of grain boundaries in polycrystalline photovoltaic semiconductors SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID FILM SOLAR-CELLS; TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; BASIS-SET; CDTE; CU(IN,GA)SE-2; PERFORMANCE; EFFICIENCY; SILICON AB Thin-film solar cells based on polycrystalline Cu(In,Ga)Se-2 (CIGS) and CdTe photovoltaic semiconductors have reached remarkable laboratory efficiencies. It is surprising that these thin-film polycrystalline solar cells can reach such high efficiencies despite containing a high density of grain boundaries (GBs), which would seem likely to be nonradiative recombination centers for photo-generated carriers. In this paper, we review our atomistic theoretical understanding of the physics of grain boundaries in CIGS and CdTe absorbers. We show that intrinsic GBs with dislocation cores exhibit deep gap states in both CIGS and CdTe. However, in each solar cell device, the GBs can be chemically modified to improve their photovoltaic properties. In CIGS cells, GBs are found to be Cu-rich and contain O impurities. Density-functional theory calculations reveal that such chemical changes within GBs can remove most of the unwanted gap states. In CdTe cells, GBs are found to contain a high concentration of Cl atoms. Cl atoms donate electrons, creating n-type GBs between p-type CdTe grains, forming local p-n-p junctions along GBs. This leads to enhanced current collections. Therefore, chemical modification of GBs allows for high efficiency polycrystalline CIGS and CdTe thin-film solar cells. (C) 2015 AIP Publishing LLC. C1 [Yan, Yanfa; Yin, Wan-Jian; Wu, Yelong; Shi, Tingting; Paudel, Naba R.; Wang, Zhiwei] Univ Toledo, Dept Phys & Astron, Toledo, OH 43606 USA. [Yan, Yanfa; Yin, Wan-Jian; Wu, Yelong; Shi, Tingting; Paudel, Naba R.; Wang, Zhiwei] Univ Toledo, Wright Ctr Photovolta Innovat & Commercializat, Toledo, OH 43606 USA. [Li, Chen] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Poplawsky, Jonathan] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Wang, Zhiwei; Moseley, John; Guthrey, Harvey; Moutinho, Helio; Al-Jassim, Mowafak M.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Pennycook, Stephen J.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. RP Yan, YF (reprint author), Univ Toledo, Dept Phys & Astron, Toledo, OH 43606 USA. EM yanfa.yan@utoledo.edu RI Wu, Yelong/G-1100-2010; Yin, Wanjian/F-6738-2013; Poplawsky, Jonathan/Q-2456-2015 OI Wu, Yelong/0000-0002-4211-911X; Poplawsky, Jonathan/0000-0002-4272-7043 FU Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; U.S. Department of Energy (DOE) Office of Energy Efficiency and Renewable Energy, Foundational Program to Advance Cell Efficiency (F-PACE); national science foundation [CHE-1230246]; U.S. Department of Energy [DE-AC36-08GO28308]; ORNL's Center for Nanophase Materials Sciences (CNMS) - Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; Ohio Research Scholar Program (ORSP) FX This research used resources of the National Energy Research Scientific Computing Center, which was supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. This work was supported by the U.S. Department of Energy (DOE) Office of Energy Efficiency and Renewable Energy, Foundational Program to Advance Cell Efficiency (F-PACE) and the national science foundation under Contract No. CHE-1230246. Work at NREL was supported by the U.S. Department of Energy under Contract No. DE-AC36-08GO28308. This work was also supported by ORNL's Center for Nanophase Materials Sciences (CNMS), which was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. The authors thank R. Noufi, I. Repins, and S.-H. Wei for proving CIGS samples and stimulating discussions. Y.Y. acknowledges the support from the Ohio Research Scholar Program (ORSP). NR 42 TC 8 Z9 8 U1 12 U2 99 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAR 21 PY 2015 VL 117 IS 11 AR 112807 DI 10.1063/1.4913833 PG 6 WC Physics, Applied SC Physics GA CE1WZ UT WOS:000351604900008 ER PT J AU Banik, S Ravichandran, L Brabec, J Hubac, I Kowalski, K Pittner, J AF Banik, Subrata Ravichandran, Lalitha Brabec, Jiri Hubac, Ivan Kowalski, Karol Pittner, Jiri TI Iterative universal state selective correction for the Brillouin-Wigner multireference coupled-cluster theory SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID QUADRUPLY EXCITED CLUSTERS; QUASI-DEGENERATE STATES; DOUBLE-EXCITATION MODEL; LOW-LYING TRIPLET; VIBRATIONAL FREQUENCIES; TETRAMETHYLENEETHANE TME; PARALLEL IMPLEMENTATION; CONTINUOUS TRANSITION; APPROXIMATE ACCOUNT; PERTURBATION-THEORY AB As a further development of the previously introduced a posteriori Universal State-Selective (USS) corrections [K. Kowalski, J. Chem. Phys. 134, 194107 (2011); J. Brabec et al., ibid. 136, 124102 (2012)], we suggest an iterative form of the USS correction by means of correcting effective Hamiltonian matrix elements. We also formulate USS corrections via the left Bloch equations. The convergence of the USS corrections with excitation level towards the full configuration interaction (FCI) limit is also investigated. Various forms of the USS and simplified diagonal USS corrections at the singles and doubles and perturbative triple levels are numerically assessed on several model systems and on the ozone and tetramethyleneethane molecules. It is shown that the iterative USS correction can successfully replace the previously developed a posteriori Brillouin-Wigner coupled cluster size-extensivity correction, while it is not sensitive to intruder states and performs well also in other cases when the a posteriori one fails, like, e. g., for the asymmetric vibration mode of ozone. (C) 2015 AIP Publishing LLC. C1 [Banik, Subrata; Ravichandran, Lalitha; Pittner, Jiri] Acad Sci Czech Republic, J Heyrovsky Inst Phys Chem, CZ-18223 Prague 8, Czech Republic. [Brabec, Jiri] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, Berkeley, CA 94720 USA. [Hubac, Ivan] Comenius Univ, Dept Chem Phys, Fac Math & Phys, Bratislava 84215, Slovakia. [Hubac, Ivan] Silesian Univ, Inst Phys, Opava 74601, Czech Republic. [Kowalski, Karol] Pacific NW Natl Lab, William R Wiley Environm Mol Sci Lab, Richland, WA 99352 USA. RP Banik, S (reprint author), Acad Sci Czech Republic, J Heyrovsky Inst Phys Chem, CZ-18223 Prague 8, Czech Republic. EM karol.kowalski@pnnl.gov; jiri.pittner@jh-inst.cas.cz FU Ministry of Education, Youth, and Sports of the Czech Republic [LH13117]; Granting Agency of the Czech Republic [208/11/2222]; VEGA grant agency [1/0530/14]; APVV grant agency [W-0420-10]; Department of Energy's Office of Biological and Environmental Research; U.S. Department of Energy by the Battelle Memorial Institute [DE-AC06-76RLO-1830]; IT4Innovations Centre of Excellence project - European Regional Development Fund [CZ.1.05/1.1.00/02.0070]; national budget of the Czech Republic via the Research and Development for Innovations Operational Programme; Czech Ministry of Education, Youth, and Sports via the project Large Research, Development, and Innovations Infrastructures [LM2011033] FX We acknowledge the support by the Ministry of Education, Youth, and Sports of the Czech Republic (Project No. LH13117) and by the Granting Agency of the Czech Republic (Project No. 208/11/2222). I.H. acknowledges the support by the VEGA grant agency (Project No. 1/0530/14) and APVV grant agency (Project No. W-0420-10). A large portion of calculations has been performed using EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. The Pacific Northwest National Laboratory is operated for the U.S. Department of Energy by the Battelle Memorial Institute under Contract No. DE-AC06-76RLO-1830. Part of the calculations has been performed at the IT4Innovations National Supercomputing Center of the VSB-Technical University of Ostrava, supported by the IT4Innovations Centre of Excellence project (CZ.1.05/1.1.00/02.0070), funded by the European Regional Development Fund and the national budget of the Czech Republic via the Research and Development for Innovations Operational Programme, as well as Czech Ministry of Education, Youth, and Sports via the project Large Research, Development, and Innovations Infrastructures (LM2011033). NR 94 TC 2 Z9 2 U1 0 U2 8 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAR 21 PY 2015 VL 142 IS 11 AR 114106 DI 10.1063/1.4914311 PG 15 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CE0WK UT WOS:000351530100006 PM 25796230 ER PT J AU Phillips, DH Watson, DB AF Phillips, D. H. Watson, D. B. TI Distribution of uranium and thorium in dolomitic gravel fill and shale saprolite SO JOURNAL OF HAZARDOUS MATERIALS LA English DT Article DE Uranium; Thorium; Amorphous basaluminite; Barite; Groundwater contamination; Oak ridge integrated field research challenge (ORIFRC) ID WEATHERED FRACTURED SAPROLITE/SHALE; EMULSIFIED VEGETABLE-OIL; CONTAMINATED GROUNDWATER; ACIDIC SEDIMENTS; ELECTRON-DONOR; BIOREDUCTION; TITRATION; SOILS; REMEDIATION; DEPOSITION AB The objectives of this study were to examine (I) the distribution of U and Th in dolomitic gravel fill and shale saprolite, and (2) the removal of uranium from acidic groundwater by dolomitic gravel through precipitation with amorphous basaluminite at the U.S. DOE Oak Ridge Integrated Field Research Challenge (ORIFRC) field site west of the Oak Ridge Y-12 National Security Complex in East Tennessee. Media reactivity and sustainability are a technical concern with the deployment of any subsurface reactive media. Because the gravel was placed in the subsurface and exposed to contaminated groundwater for over 20 years, it provided a unique opportunity to study the solid and water phase geochemical conditions within the media after this length of exposure. This study illustrates that dolomite gravel can remove U from acidic contaminated groundwater with high levels of Al3+, Ca2+, NO3-, and SO42- over the long term. As the groundwater flows through high pH carbonate gravel, U containing amorphous basaluminite precipitates as the pH increases. This is due to an increase in groundwater pH from 3.2 to similar to 6.5 as it comes in contact with the gravel. Therefore, carbonate gravel could be considered as a possible treatment medium for removal and sequestration of U and other pH sensitive metals from acidic contaminated groundwater. Thorium concentrations are also high in the carbonate gravel. Thorium generally shows an inverse relationship with U from the surface down into the deeper saprolite. Barite precipitated in the shallow saprolite directly below the dolomitic gravel from barium present in the acidic contaminated groundwater. (C) 2014 Elsevier B.V. All rights reserved. C1 [Phillips, D. H.] Queens Univ Belfast, Environm Engn Res Ctr, Sch Planning Architecture & Civil Engn, Belfast BT9 5AG, Antrim, North Ireland. [Watson, D. B.] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. RP Watson, DB (reprint author), Oak Ridge Natl Lab, Div Environm Sci, POB 2008, Oak Ridge, TN 37831 USA. EM watsondb@orn1.gov RI Phillips, Debra/F-1828-2010; Watson, David/C-3256-2016 OI Phillips, Debra/0000-0001-8548-7409; Watson, David/0000-0002-4972-4136 FU U.S. DOE, Office of Science, Office of Biological and Environmental Research (BER), Subsurface Biogeochemical Research Program; U.S. DOE [DE-AC05-18 00OR22725] FX This research was funded by the U.S. DOE, Office of Science, Office of Biological and Environmental Research (BER), Subsurface Biogeochemical Research Program. Oak Ridge National Laboratory is managed by UT-Battelle, LLC, for the U.S. DOE under contract DE-AC05-18 00OR22725. The authors also thank Kenneth Lowe and Tonia Mehlhorn for assistance with the sampling and analysis. NR 27 TC 1 Z9 1 U1 0 U2 17 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0304-3894 EI 1873-3336 J9 J HAZARD MATER JI J. Hazard. Mater. PD MAR 21 PY 2015 VL 285 BP 474 EP 482 DI 10.1016/j.jhazmat.2014.11.046 PG 9 WC Engineering, Environmental; Engineering, Civil; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA CB8LC UT WOS:000349880100058 PM 25544493 ER PT J AU Ruz, J Brejnholt, NF Alameda, JB Decker, TA Descalle, MA Fernandez-Perea, M Hill, RM Kisner, RA Melin, AM Patton, BW Soufli, R Ziock, K Pivovaroff, MJ AF Ruz, J. Brejnholt, N. F. Alameda, J. B. Decker, T. A. Descalle, M. A. Fernandez-Perea, M. Hill, R. M. Kisner, R. A. Melin, A. M. Patton, B. W. Soufli, R. Ziock, K. Pivovaroff, M. J. TI Direct measurement of U-235 in spent fuel rods with Gamma-ray mirrors SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Fission; Spent fuel; Non-destructive analysis; X-ray fluorescence; Uranium quantification; Gamma-ray mirrors AB Direct measurement of plutonium and uranium X-rays and gamma-rays is a highly desirable nondestructive analysis method for the use in reprocessing fuel environments. The high background and intense radiation from spent fuel make direct measurements difficult to implement since the relatively low activity of uranium and plutonium is masked by the high activity from fission products. To overcome this problem, we make use of a grazing incidence optic to selectively reflect K-alpha and K-beta fluorescence of Special Nuclear Materials (SNM) into a high-purity position-sensitive germanium detector and obtain their relative ratios. (C) 2014 Elsevier B.V. All rights reserved. C1 [Ruz, J.; Brejnholt, N. F.; Alameda, J. B.; Decker, T. A.; Descalle, M. A.; Fernandez-Perea, M.; Hill, R. M.; Soufli, R.; Pivovaroff, M. J.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Kisner, R. A.; Melin, A. M.; Patton, B. W.; Ziock, K.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Ruz, J (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM ruzarmendari1@llnl.gov FU Lawrence Livermore National Security, LLC [DE-AC52-07NA27344]; U.S. Department of Energy FX This paper has been authored by Lawrence Livermore National Security, LLC under Contract no. DE-AC52-07NA27344 with U.S. Department of Energy. NR 11 TC 1 Z9 1 U1 0 U2 12 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD MAR 21 PY 2015 VL 777 BP 15 EP 19 DI 10.1016/j.nima.2014.12.055 PG 5 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CB2PB UT WOS:000349468800003 ER PT J AU Gorgen, P Boine-Frankenheim, O Fischer, W AF Goergen, P. Boine-Frankenheim, O. Fischer, W. TI Beam transfer functions for relativistic proton bunches with beam-beam interaction SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Beam transfer function; Tune distribution; Electron lens; Incoherent effects; Hadron colliders; Beam-beam AB We present a method for the recovery of the Lransverse tune spread directly from the beam transfer Function (BTF). The model is applicable for coasting beams and bunched beams at high energy with a tune spread from transverse nonlinearities induced by the beam-beam effect or by an electron lens. Other sources of tune spread can be added. A method for the recovery of the incoherent tune spread without prior knowledge of the nonlinearity is presented. The approach is based on the analytic model for BTFs of coasting beams, which agrees very well with simulations results for bunched beams at relativistic energies with typically low synchrotron tune. A priori the presented tune spread recovery method is usable only in the absence of coherent modes, but additional simulation data shows its applicability even in the presence of coherent beam-beam modes. Finally agreement of both he analytic and simulation models with measurement data obtained at REUC is presented. The proposed method successfully recovers the tune spread from analytic, simulated and measured BIT. (C) 2014 Elsevier By. All rights reserved. C1 [Goergen, P.; Boine-Frankenheim, O.] Tech Univ Darmstadt, Inst Theorie Elektromagnet Felder TEMF, D-64289 Darmstadt, Germany. [Fischer, W.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Gorgen, P (reprint author), Tech Univ Darmstadt, Inst Theorie Elektromagnet Felder TEMF, Schlossgartenstr 8, D-64289 Darmstadt, Germany. EM goergen@temf.tu-darmstadt.de OI Boine-Frankenheim, Oliver/0000-0002-3225-078X FU U.S. DOE [DE-AC02-98CH10886]; U.S. Department of Energy FX P. Gorgen wishes to thank S. White for his support with the measurements and the implementation of beam-beam in the simulation code and M. Blaskiewicz for helpful discussions dur-ing the implementation of beam-beam and BTF, especially during implementation of the averaging method for white noise BTF. Work was supported in part by U.S. DOE under Contract no DE-AC02-98CH10886 with the U.S. Department of Energy. NR 19 TC 2 Z9 2 U1 0 U2 1 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD MAR 21 PY 2015 VL 777 BP 43 EP 53 DI 10.1016/j.nima.2014.11.105 PG 11 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CB2PB UT WOS:000349468800007 ER PT J AU Battaglieri, M Boyarinov, S Bueltmann, S Burkert, V Celentano, A Charles, G Cooper, W Cuevas, C Dashyan, N DeVita, R Desnault, C Deur, A Egiyan, H Elouadrhiri, L Essig, R Fadeyev, V Field, C Freyberger, A Gershtein, Y Gevorgyan, N Girod, FX Graf, N Graham, M Griffioen, K Grillo, A Guidal, M Haller, G Adrian, PH Herbst, R Holtrop, M Jaros, J Kaneta, S Khandaker, M Kubarovsky, A Kubarovsky, V Maruyama, T McCormick, J Moffeit, K Moreno, O Neal, H Nelson, T Niccolai, S Odian, A Oriunno, M Paremuzyan, R Partridge, R Phillips, SK Rauly, E Raydo, B Reichert, J Rindel, E Rosier, P Salgado, C Schuster, P Sharabian, Y Sokhan, D Stepanyan, S Toro, N Uemura, S Ungaro, M Voskanyan, H Walz, D Weinstein, LB Wojtsekhowski, B AF Battaglieri, M. a Boyarinov, S. b Bueltmann, S. c Burkert, V. b Celentano, A. a Charles, G. f Cooper, W. d Cuevas, C. b Dashyan, N. e DeVita, R. a Desnault, C. f Deur, A. b Egiyan, H. b Elouadrhiri, L. b Essig, R. g Fadeyev, V. h Field, C. i Freyberger, A. b Gershtein, Y. j Gevorgyan, N. e Girod, F. -X. b Graf, N. i Graham, M. i Griffioen, K. k Grillo, A. h Guidal, M. f Haller, G. i Adrian, P. Hansson i Herbst, R. i Holtrop, M. l Jaros, J. i Kaneta, S. b Khandaker, M. m Kubarovsky, A. n Kubarovsky, V. b Maruyama, T. i McCormick, J. i Moffeit, K. i Moreno, O. h Neal, H. i Nelson, T. i Niccolai, S. f Odian, A. i Oriunno, M. i Paremuzyan, R. e Partridge, R. i Phillips, S. K. l Rauly, E. f Raydo, B. b Reichert, J. j Rindel, E. f Rosier, P. f Salgado, C. m Schuster, P. o Sharabian, Y. b Sokhan, D. p Stepanyan, S. b Toro, N. o Uemura, S. i Ungaro, M. b Voskanyan, H. e Walz, D. i Weinstein, L. B. c Wojtsekhowski, B. b TI The Heavy Photon Search test detector SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Silicon; Tracking; Vertexing; Heavy photon; Dark photon; Electromagnetic calorimeter ID FRONT-END CHIP; INFORMATION; APV25 AB The Heavy Photon Search (HPS), an experiment to search for a hidden sector photon in fixed target electroproduction, is preparing for installation at the Thomas Jefferson National Accelerator Facility (JLab) in the Fall of 2014. As the first stage of this project, the HPS Test Run apparatus was constructed and operated in 2012 to demonstrate the experiment's technical feasibility and to confirm that the trigger rates and occupancies are as expected. This paper describes the HPS Test Run apparatus and readout electronics and its performance. In this setting, a heavy photon can be identified as a narrow peak in the e(+)e(-) invariant mass spectrum above the trident background or as a narrow invariant mass peak with a decay vertex displaced from the production target, so charged particle tracking and vertexing are needed for its detection. In the HPS Test Run, charged particles are measured with a compact forward silicon microstrip tracker inside a dipole magnet. Electromagnetic showers are detected in a PbW0(4) crystal calorimeter situated behind the magnet, and are used to trigger the experiment and identify electrons and positrons. Both detectors are placed close to the beam line and split top bottom. This arrangement provides sensitivity to low mass heavy photons, allows clear passage of the unscattered beam, and avoids the spray of degraded electrons coming from the target. The discrimination between prompt and displaced e(+)e(-) pairs requires the first layer of silicon sensors be placed only 10 cm downstream of the target. The expected signal is small, and the trident background huge, so the experiment requires very large statistics. Accordingly, the HPS Test Run utilizes high-rate readout and data acquisition electronics and a fast trigger to exploit the essentially 100% duty cycle of the CEBAF accelerator at JLab. (C) 2014 The Authors. Published by Elsevier B.V. C1 [Battaglieri, M. a; Celentano, A. a] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Battaglieri, M. a; Celentano, A. a] Ist Nazl Fis Nucl, Dipartimento Fis, I-16146 Genoa, Italy. [Boyarinov, S. b; Burkert, V. b; Cuevas, C. b; Deur, A. b; Egiyan, H. b; Elouadrhiri, L. b; Freyberger, A. b; Girod, F. -X. b; Kaneta, S. b; Kubarovsky, V. b; Raydo, B. b; Sharabian, Y. b; Stepanyan, S. b; Ungaro, M. b; Wojtsekhowski, B. b] Thomas Jefferson Natl Accelerator Fac, Newport News, VA 23606 USA. [Bueltmann, S. c; Weinstein, L. B. c] Old Dominion Univ, Norfolk, VA 23529 USA. [Cooper, W. d] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Dashyan, N. e; Gevorgyan, N. e; Paremuzyan, R. e; Voskanyan, H. e] Yerevan Phys Inst, Yerevan 375036, Armenia. [Charles, G. f; Desnault, C. f; Guidal, M. f; Niccolai, S. f; Rauly, E. f; Rindel, E. f; Rosier, P. f] Univ Paris 11, Inst Phys Nucl, Orsay, France. [Charles, G. f; Desnault, C. f; Guidal, M. f; Niccolai, S. f; Rauly, E. f; Rindel, E. f; Rosier, P. f] CNRS, IN2P3, F-91405 Orsay, France. [Essig, R. g] SUNY Stony Brook, Stony Brook, NY 11794 USA. [Fadeyev, V. h; Grillo, A. h; Moreno, O. h] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Field, C. i; Graf, N. i; Graham, M. i; Haller, G. i; Herbst, R. i; Jaros, J. i; Maruyama, T. i; McCormick, J. i; Moffeit, K. i; Neal, H. i; Nelson, T. i; Odian, A. i; Oriunno, M. i; Partridge, R. i; Uemura, S. i; Walz, D. i] SLAC, Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Gershtein, Y. j; Reichert, J. j] Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08854 USA. [Griffioen, K. k] Coll William & Mary, Dept Phys, Williamsburg, VA 23185 USA. [Holtrop, M. l; Phillips, S. K. l] Univ New Hampshire, Dept Phys, Durham, NH 03824 USA. [Khandaker, M. m; Salgado, C. m] Norfolk State Univ, Norfolk, VA 23504 USA. [Kubarovsky, A. n] Rensselaer Polytech Inst, Dept Phys, Troy, NY 12181 USA. [Schuster, P. o; Toro, N. o] Perimeter Inst, Waterloo, ON N2L 2Y5, Canada. [Sokhan, D. p] Univ Glasgow, Glasgow G12 8QQ, Lanark, Scotland. RP Adrian, PH (reprint author), SLAC, Natl Accelerator Lab, Menlo Pk, CA 94025 USA. EM phansson@slac.stanford.edu RI Celentano, Andrea/J-6190-2012 OI Celentano, Andrea/0000-0002-7104-2983 FU U.S. Department of Energy [DE-AC02-76SF00515, DE-AC05-06OR23177]; National Science Foundation; French Centre National de la Recherche Scientifique; Italian Istituto Nazionale di Fisica Nucleare; Department of Energy Early Career research program [DESC0008061]; Sloan Foundation Research Fellowship FX Work supported by the U.S. Department of Energy under contract number DE-AC02-76SF00515, the National Science Foundation, French Centre National de la Recherche Scientifique and Italian Istituto Nazionale di Fisica Nucleare. Rouven Essig is supported in part by the Department of Energy Early Career research program DESC0008061 and by a Sloan Foundation Research Fellowship. Authored by Jefferson Science Associates, LLC under U.S. Department of Energy contract No. DE-AC05-06OR23177. NR 20 TC 10 Z9 10 U1 0 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD MAR 21 PY 2015 VL 777 BP 91 EP 101 DI 10.1016/j.nima.2014.12.017 PG 11 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CB2PB UT WOS:000349468800014 ER PT J AU Looker, Q Amman, M Vetter, K AF Looker, Q. Amman, M. Vetter, K. TI Leakage current in high-purity germanium detectors with amorphous semiconductor contacts SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Gamma-ray detectors; High-parity germanium; Radiation detectors; Semiconductor radiation detectors ID ORTHOGONAL-STRIP DETECTORS; BLOCKING CONTACTS; RAY-DETECTORS; GE DETECTORS; SILICON; SPECTROSCOPY; FILMS; FABRICATION; OPERATION; BARRIER AB Amorphous semiconductor electrical contacts on high purity Ge radiation detectors have become a valuable technology because they are simple to fabricate, result in thin dead layers, block both electron and hole injection, and can readily be finely segmented as needed for applications requiring imaging or particle tracking. Though significant numbers of detectors have been successfully produced for a variety of applications using the amorphous semiconductor contact technology, there remains a need to better understand the dependence of performance characteristics, particularly leakage current, on the fabrication process parameters so that the performance can be better optimized. To this end, we have performed a systematic study of leakage current on BF-sputter-deposited amorphous-Ge (a-Ge) and amorphous-Si (a-Si) contacts as a function of process and operational parameters including sputter gas pressure and composition, number of detector temperature cycles, and time spent at room temperature. The study focused primarily on the current resulting from electron injection at the contact. Significant findings from the study include that a-Si produces lower electron injection than a-Ge, the time the detector spends at room temperature rather than the number of temperature cycles experienced by the detector is the primary factor associated with leakage current change when the detector is warmed, and the time stability of the a-Ge contact depends on the sputter gas pressure with a higher pressure producing more stable characteristics. (C) 2015 Elsevier B.V. All rights reserved. C1 [Looker, Q.; Amman, M.; Vetter, K.] Univ Calif Berkeley, Ernest Orlando Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Looker, Q.; Vetter, K.] Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA. RP Looker, Q (reprint author), Univ Calif Berkeley, Ernest Orlando Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM qlooker@lbl.gov FU U.S. Department of Energy, Office of Science [DE-AC02-05CH11231] FX We thank Paul Luke for useful discussions throughout this project, This work was supported by the U.S. Department of Energy, Office of Science, under contract number DE-AC02-05CH11231. NR 55 TC 2 Z9 2 U1 0 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD MAR 21 PY 2015 VL 777 BP 138 EP 147 DI 10.1016/j.nima.2014.12.104 PG 10 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CB2PB UT WOS:000349468800020 ER PT J AU Whitelam, S Tamblyn, I Garrahan, JP Beton, PH AF Whitelam, Stephen Tamblyn, Isaac Garrahan, Juan P. Beton, Peter H. TI Emergent Rhombus Tilings from Molecular Interactions with M-fold Rotational Symmetry SO PHYSICAL REVIEW LETTERS LA English DT Article ID CRYSTALLIZATION; TRANSITIONS; SURFACES AB We show that model molecules with particular rotational symmetries can self-assemble into network structures equivalent to rhombus tilings. This assembly happens in an emergent way, in the sense that molecules spontaneously select irregular fourfold local coordination from a larger set of possible local binding geometries. The existence of such networks can be rationalized by simple geometrical arguments, but the same arguments do not guarantee a network's spontaneous self-assembly. This class of structures must in certain regimes of parameter space be able to reconfigure into networks equivalent to triangular tilings. C1 [Whitelam, Stephen] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Tamblyn, Isaac] Univ Ontario, Dept Phys, Inst Technol, Oshawa, ON L1H 7K4, Canada. [Garrahan, Juan P.; Beton, Peter H.] Univ Nottingham, Sch Phys & Astron, Nottingham NG7 2RD, England. RP Whitelam, S (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM swhitelam@lbl.gov RI Foundry, Molecular/G-9968-2014; Beton, Peter/M-5303-2014 OI Garrahan, Juan/0000-0002-0185-3924; Tamblyn, Isaac/0000-0002-8146-6667; Beton, Peter/0000-0002-2120-8033 FU Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; EPSRC [EP/K01773X/1]; NSERC FX This work was done as part of a User Project at the Molecular Foundry, Lawrence Berkeley National Laboratory, supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. J.P.G. and P.H.B. acknowledge support from EPSRC Grant No. EP/K01773X/1. I.T. acknowledges support from NSERC. NR 45 TC 3 Z9 3 U1 0 U2 16 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 20 PY 2015 VL 114 IS 11 AR 115702 DI 10.1103/PhysRevLett.114.115702 PG 5 WC Physics, Multidisciplinary SC Physics GA CE8DY UT WOS:000352072800012 PM 25839291 ER PT J AU Chapman, C Henry, M Bishop-Lilly, KA Awosika, J Briska, A Ptashkin, RN Wagner, T Rajanna, C Tsang, H Johnson, SL Mokashi, VP Chain, PSG Sozhamannan, S AF Chapman, Carol Henry, Matthew Bishop-Lilly, Kimberly A. Awosika, Joy Briska, Adam Ptashkin, Ryan N. Wagner, Trevor Rajanna, Chythanya Tsang, Hsinyi Johnson, Shannon L. Mokashi, Vishwesh P. Chain, Patrick S. G. Sozhamannan, Shanmuga TI Scanning the Landscape of Genome Architecture of Non-O1 and Non-O139 Vibrio cholerae by Whole Genome Mapping Reveals Extensive Population Genetic Diversity SO PLOS ONE LA English DT Article ID STRAINS; EPIDEMIC; EMERGENCE; REGIONS; HAITI AB Historically, cholera outbreaks have been linked to V. cholerae O1 serogroup strains or its derivatives of the O37 and O139 serogroups. A genomic study on the 2010 Haiti cholera outbreak strains highlighted the putative role of non O1/non-O139 V. cholerae in causing cholera and the lack of genomic sequences of such strains from around the world. Here we address these gaps by scanning a global collection of V. cholerae strains as a first step towards understanding the population genetic diversity and epidemic potential of non O1/non-O139 strains. Whole Genome Mapping (Optical Mapping) based bar coding produces a high resolution, ordered restriction map, depicting a complete view of the unique chromosomal architecture of an organism. To assess the genomic diversity of non-O1/non-O139 V. cholerae, we applied a Whole Genome Mapping strategy on a well-defined and geographically and temporally diverse strain collection, the Sakazaki serogroup type strains. Whole Genome Map data on 91 of the 206 serogroup type strains support the hypothesis that V. cholerae has an unprecedented genetic and genomic structural diversity. Interestingly, we discovered chromosomal fusions in two unusual strains that possess a single chromosome instead of the two chromosomes usually found in V. cholerae. We also found pervasive chromosomal rearrangements such as duplications and indels in many strains. The majority of Vibrio genome sequences currently in public databases are unfinished draft sequences. The Whole Genome Mapping approach presented here enables rapid screening of large strain collections to capture genomic complexities that would not have been otherwise revealed by unfinished draft genome sequencing and thus aids in assembling and finishing draft sequences of complex genomes. Furthermore, Whole Genome Mapping allows for prediction of novel V. cholerae non-O1/non-O139 strains that may have the potential to cause future cholera outbreaks. C1 [Chapman, Carol; Henry, Matthew; Bishop-Lilly, Kimberly A.; Awosika, Joy; Tsang, Hsinyi; Sozhamannan, Shanmuga] Henry M Jackson Fdn, Bethesda, MD USA. [Chapman, Carol; Henry, Matthew; Bishop-Lilly, Kimberly A.; Awosika, Joy; Tsang, Hsinyi; Mokashi, Vishwesh P.; Sozhamannan, Shanmuga] Naval Med Res Ctr Frederick, Ft Detrick, MD USA. [Briska, Adam; Ptashkin, Ryan N.; Wagner, Trevor] OpGen Inc, Gaithersburg, MD USA. [Rajanna, Chythanya] Univ Florida, Gainesville, FL USA. [Johnson, Shannon L.; Chain, Patrick S. G.] Los Alamos Natl Lab, Biosci Div, Genome Sci, Los Alamos, NM USA. RP Sozhamannan, S (reprint author), GoldBelt Raven LLC, Frederick, MD 21701 USA. EM Shanmuga.Sozhamannan.ctr@mail.mil OI Chain, Patrick/0000-0003-3949-3634 FU Defense Threat Reduction Agency [TMTI_IB06RSQ002] FX This work was supported under contract TMTI_IB06RSQ002 through the Defense Threat Reduction Agency to SS. Additional support was provided by OpGen, Inc for data collection, analyses and interpretation of data. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 25 TC 1 Z9 1 U1 0 U2 7 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAR 20 PY 2015 VL 10 IS 3 AR e0120311 DI 10.1371/journal.pone.0120311 PG 15 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CE8HY UT WOS:000352083900010 PM 25794000 ER PT J AU Engler, RJM Nelson, MR Collins, LC Spooner, C Hemann, BA Gibbs, BT Atwood, JE Howard, RS Chang, AS Cruser, DL Gates, DG Vernalis, MN Lengkeek, MS McClenathan, BM Jaffe, AS Cooper, LT Black, S Carlson, C Wilson, C Davis, RL AF Engler, Renata J. M. Nelson, Michael R. Collins, Limone C., Jr. Spooner, Christina Hemann, Brian A. Gibbs, Barnett T. Atwood, J. Edwin Howard, Robin S. Chang, Audrey S. Cruser, Daniel L. Gates, Daniel G. Vernalis, Marina N. Lengkeek, Marguerite S. McClenathan, Bruce M. Jaffe, Allan S. Cooper, Leslie T. Black, Steve Carlson, Christopher Wilson, Christopher Davis, Robert L. TI A Prospective Study of the Incidence of Myocarditis/Pericarditis and New Onset Cardiac Symptoms following Smallpox and Influenza Vaccination SO PLOS ONE LA English DT Article ID INDUCED MYOCARDIAL-ISCHEMIA; LONG-TERM MORTALITY; TROPONIN-T; ADVERSE EVENTS; UNITED-STATES; GENERAL-POPULATION; RISK; ELEVATION; EXERCISE; RECOMMENDATIONS AB Background Although myocarditis/pericarditis (MP) has been identified as an adverse event following smallpox vaccine (SPX), the prospective incidence of this reaction and new onset cardiac symptoms, including possible subclinical injury, has not been prospectively defined. Purpose The study's primary objective was to determine the prospective incidence of new onset cardiac symptoms, clinical and possible subclinical MP in temporal association with immunization. Methods New onset cardiac symptoms, clinical MP and cardiac specific troponin T (cTnT) elevations following SPX (above individual baseline values) were measured in a multi-center prospective, active surveillance cohort study of healthy subjects receiving either smallpox vaccine or trivalent influenza vaccine (TIV). Results New onset chest pain, dyspnea, and/or palpitations occurred in 10.6% of SPX-vaccinees and 2.6% of TIV-vaccinees within 30 days of immunization (relative risk (RR) 4.0, 95% CI: 1.7-9.3). Among the 1081 SPX-vaccinees with complete follow-up, 4 Caucasian males were diagnosed with probable myocarditis and 1 female with suspected pericarditis. This indicates a post-SPX incidence rate more than 200-times higher than the pre-SPX background population surveillance rate of myocarditis/pericarditis (RR 214, 95% CI 65-558). Additionally, 31 SPX-vaccinees without specific cardiac symptoms were found to have over 2-fold increases in cTnT (>99th percentile) from baseline (pre-SPX) during the window of risk for clinical myocarditis/pericarditis and meeting a proposed case definition for possible subclinical myocarditis. This rate is 60-times higher than the incidence rate of overt clinical cases. No clinical or possible subclinical myocarditis cases were identified in the TIV-vaccinated group. Conclusions Passive surveillance significantly underestimates the true incidence of myocarditis/pericarditis after smallpox immunization. Evidence of subclinical transient cardiac muscle injury post-vaccinia immunization is a finding that requires further study to include long-term outcomes surveillance. Active safety surveillance is needed to identify adverse events that are not well understood or previously recognized. C1 [Engler, Renata J. M.; Collins, Limone C., Jr.; Spooner, Christina] Walter Reed Natl Mil Med Ctr, Immunizat Healthcare Branch, Def Hlth Agcy, Mil Vaccine Agcy Vaccine Healthcare Ctr Network, Bethesda, MD 20889 USA. [Engler, Renata J. M.; Nelson, Michael R.] Uniformed Serv Univ Hlth Sci, Dept Med & Pediat, Bethesda, MD 20814 USA. [Nelson, Michael R.] Walter Reed Natl Mil Med Ctr, Allergy Immunol Immunizat, Bethesda, MD USA. [Hemann, Brian A.; Gibbs, Barnett T.; Atwood, J. Edwin] Walter Reed Natl Mil Med Ctr, Dept Med, Serv Cardiol, Bethesda, MD USA. [Hemann, Brian A.; Gibbs, Barnett T.; Atwood, J. Edwin] Uniformed Serv Univ Hlth Sci, Dept Med, Bethesda, MD 20814 USA. [Howard, Robin S.; Chang, Audrey S.] Walter Reed Natl Mil Med Ctr, Dept Res Programs, Bethesda, MD USA. [Cruser, Daniel L.] Vassar Bros Med Ctr, Dept Pathol, Poughkeepsie, NY USA. [Gates, Daniel G.] Ft Belvoir Community Hosp, Serv Cardiol, Ft Belvoir, VA USA. [Vernalis, Marina N.] Walter Reed Natl Mil Med Ctr, Integrated Cardiac Hlth Project, Bethesda, MD USA. [Lengkeek, Marguerite S.] Allergy & Asthma Care Ctr, Chantilly, VA USA. [McClenathan, Bruce M.] Womack Army Med Ctr, Def Hlth Agcy, Immunizat Healthcare Branch, Mil Vaccine Agcy Vaccine Healthcare Ctr Network, Ft Bragg, NC USA. [Jaffe, Allan S.; Cooper, Leslie T.] Mayo Clin, Div Cardiovasc Dis, Rochester, MN USA. [Black, Steve] Cincinnati Childrens Hosp Ctr Global Hlth, Cincinnati, OH USA. [Carlson, Christopher] Fred Hutchinson Canc Res Ctr, Div Publ Hlth Sci, Seattle, WA 98104 USA. [Wilson, Christopher] Univ Washington, Dept Immunol, Seattle, WA 98195 USA. [Davis, Robert L.] Univ Tennessee, Ctr Hlth Sci, Ctr Biomed Informat, Memphis, TN 38163 USA. [Davis, Robert L.] Oak Ridge Natl Lab, Oak Ridge, TN USA. RP Engler, RJM (reprint author), Walter Reed Natl Mil Med Ctr, Immunizat Healthcare Branch, Def Hlth Agcy, Mil Vaccine Agcy Vaccine Healthcare Ctr Network, Bethesda, MD 20889 USA. EM renata.engler@gmail.com FU Centers for Disease Control and Prevention [200-2002-00732]; National Institute of Allergy and Infectious Disease Population Genetics Program [N01 AI40069]; Federal funds from the National Institute of Allergies and Infectious Diseases, National Institutes of Health, Department of Health and Human Services [HHSN272201000024C] FX This study was supported by the Vaccine Healthcare Centers Network and Allergy-Immunology, Walter Reed Army Medical Center (Bethesda, MD)/Military Vaccine Agency, Office of the Army Surgeon General, Clinical Immunization Safety Assessment Network (Atlanta, GA) (subcontract with America's Health Insurance Plans under contract 200-2002-00732 from the Centers for Disease Control and Prevention), National Institute of Allergy and Infectious Disease Population Genetics Program (N01 AI40069). This project has been funded in part with Federal funds from the National Institute of Allergies and Infectious Diseases, National Institutes of Health, Department of Health and Human Services, under Contract No. HHSN272201000024C. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 50 TC 5 Z9 5 U1 0 U2 6 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAR 20 PY 2015 VL 10 IS 3 AR e0118283 DI 10.1371/journal.pone.0118283 PG 18 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CE8IA UT WOS:000352084200018 PM 25793705 ER PT J AU Zhang, X Lei, DS Zhang, L Rames, M Zhang, SL AF Zhang, Xing Lei, Dongsheng Zhang, Lei Rames, Matthew Zhang, Shengli TI A Model of Lipid-Free Apolipoprotein A-I Revealed by Iterative Molecular Dynamics Simulation SO PLOS ONE LA English DT Article ID HIGH-DENSITY-LIPOPROTEINS; RESONANCE ENERGY-TRANSFER; COMPUTATIONAL-EXPERIMENTAL-APPROACH; STRUCTURAL ORGANIZATION; APOA-I; SECONDARY STRUCTURE; FLUORESCENCE PROBE; DOMAIN-STRUCTURE; STABILITY; CONFORMATION AB Apolipoprotein A-I (apo A-I), the major protein component of high-density lipoprotein, has been proven inversely correlated to cardiovascular risk in past decades. The lipid-free state of apo A-I is the initial stage which binds to lipids forming high-density lipoprotein. Molecular models of lipid-free apo A-I have been reported by methods like X-ray crystallography and chemical cross-linking/mass spectrometry (CCL/MS). Through structural analysis we found that those current models had limited consistency with other experimental results, such as those from hydrogen exchange with mass spectrometry. Through molecular dynamics simulations, we also found those models could not reach a stable equilibrium state. Therefore, by integrating various experimental results, we proposed a new structural model for lipidfree apo A-I, which contains a bundled four-helix N-terminal domain (1-192) that forms a variable hydrophobic groove and a mobile short hairpin C-terminal domain (193-243). This model exhibits an equilibrium state through molecular dynamics simulation and is consistent with most of the experimental results known from CCL/MS on lysine pairs, fluorescence resonance energy transfer and hydrogen exchange. This solution-state lipid-free apo A-I model may elucidate the possible conformational transitions of apo A-I binding with lipids in high-density lipoprotein formation. C1 [Zhang, Xing; Lei, Dongsheng; Zhang, Shengli] Xi An Jiao Tong Univ, Dept Appl Phys, Xian 710049, Shaanxi, Peoples R China. [Zhang, Xing; Lei, Dongsheng; Zhang, Lei; Rames, Matthew] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Mol Foundry, Berkeley, CA 94720 USA. RP Zhang, SL (reprint author), Xi An Jiao Tong Univ, Dept Appl Phys, Xian 710049, Shaanxi, Peoples R China. EM zhangsl@mail.xjtu.edu.cn RI Foundry, Molecular/G-9968-2014; Zhang, Lei/G-6427-2012 OI Zhang, Lei/0000-0002-4880-824X FU National Nature Science Foundation of China [11374237] FX The research was funded by National Nature Science Foundation of China (No. 11374237). The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 61 TC 1 Z9 1 U1 0 U2 6 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAR 20 PY 2015 VL 10 IS 3 AR e0120233 DI 10.1371/journal.pone.0120233 PG 15 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CE8IA UT WOS:000352084200164 PM 25793886 ER PT J AU Etampawala, T Ratnaweera, D Morgan, B Diallo, S Mamontov, E Dadmun, M AF Etampawala, Thusitha Ratnaweera, Dilru Morgan, Brian Diallo, Souleymane Mamontov, Eugene Dadmun, Mark TI Monitoring the dynamics of miscible P3HT:PCBM blends: A quasi elastic neutron scattering study of organic photovoltaic active layers SO POLYMER LA English DT Article DE Organic photovoltaic; Neutron scattering; Dynamics ID POLYMER-FULLERENE BLENDS; SOLAR-CELLS; THIN-FILMS; MORPHOLOGY; POLY(3-HEXYLTHIOPHENE); NMR; MISCIBILITY; TRANSITIONS; BEHAVIOR; MODEL AB This work addresses the detailed molecular dynamic behavior of miscible blends of Poly(3-hexylthiophene) (P3HT) and [6,6]-phenyl-C61-butyric acid methyl ester (PCBM) and their pure counterparts by quasi-elastic neutron scattering measurements (QENS). The study provides the measure of relaxation processes on pico-to-nanosecond time scales. A single relaxation process was observed in pure P3HT and PCBM while two relaxation processes, one fast and one slow, were observed in the blends. The fast process was attributed to the dynamics of P3HT while the slow process was correlated to the dynamics of PCBM. The results show that the relaxation process is a balance between two opposing effects: increased mobility due to thermal activation of P3HT molecules and decrease mobility due to the presence of PCBM which is correlated to the percent crystallinity of P3HT and local packing density of PCBM in the amorphous phase. The threshold for the domination of the thermally activated relaxation is between 5 and 9 vol.% of PCBM loading. Two distinct spatial dependences of the relaxation processes, in which the crossover length scale depends neither on temperature nor composition, were observed for all the samples. They were attributed to the collective motions of the hexyl side chains and the rotational motions of the C-C single bonds of the side chains. These results provide an understanding of the effects of PCBM loading and temperature on the dynamics of the polymer-fullerene blends which provides a tool to optimize the efficiency of charge carrier and exciton transport within the organic photovoltaic (OPV) active layer to improve the high performance of organic solar cells. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Etampawala, Thusitha; Ratnaweera, Dilru; Morgan, Brian; Dadmun, Mark] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Diallo, Souleymane] Oak Ridge Natl Lab, Quantum Condensed Mat Div, Oak Ridge, TN 37831 USA. [Mamontov, Eugene] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. [Dadmun, Mark] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. RP Dadmun, M (reprint author), Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. EM Dad@utk.edu RI Mamontov, Eugene/Q-1003-2015; Diallo, Souleymane/B-3111-2016 OI Mamontov, Eugene/0000-0002-5684-2675; Diallo, Souleymane/0000-0002-3369-8391 FU Sustainable Energy Education Research Center; Joint Institute for Neutron Sciences at the University of Tennessee; National Science Foundation [DMR-1005987]; Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy FX The authors wish to acknowledge the Sustainable Energy Education Research Center and the Joint Institute for Neutron Sciences at the University of Tennessee, as well as the National Science Foundation (DMR-1005987) for support of this project. MDD also acknowledges the support of the Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. The quasi-elastic neutron scattering measurements conducted using the BASIS at ORNL's Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. NR 37 TC 2 Z9 2 U1 1 U2 20 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0032-3861 EI 1873-2291 J9 POLYMER JI Polymer PD MAR 20 PY 2015 VL 61 BP 155 EP 162 DI 10.1016/j.polymer.2015.01.064 PG 8 WC Polymer Science SC Polymer Science GA CE8TY UT WOS:000352118200019 ER PT J AU Grefenstette, BW Reynolds, SP Harrison, FA Humensky, TB Boggs, SE Fryer, CL DeLaney, T Madsen, KK Miyasaka, H Wik, DR Zoglauer, A Forster, K Kitaguchi, T Lopez, L Nynka, M Christensen, FE Craig, WW Hailey, CJ Stern, D Zhang, WW AF Grefenstette, Brian W. Reynolds, Stephen P. Harrison, Fiona A. Humensky, T. Brian Boggs, Steven E. Fryer, Chris L. DeLaney, Tracey Madsen, Kristin K. Miyasaka, Hiromasa Wik, Daniel R. Zoglauer, Andreas Forster, Karl Kitaguchi, Takao Lopez, Laura Nynka, Melania Christensen, Finn E. Craig, William W. Hailey, Charles J. Stern, Daniel Zhang, William W. TI LOCATING THE MOST ENERGETIC ELECTRONS IN CASSIOPEIA A SO ASTROPHYSICAL JOURNAL LA English DT Article DE acceleration of particles; ISM: individual objects (Cassiopeia A); ISM: supernova remnants; radiation mechanisms: non-thermal; X-rays: ISM ID SUPERNOVA REMNANT CASSIOPEIA; X-RAY-EMISSION; PARTICLE-ACCELERATION; SYNCHROTRON EMISSION; MAGNETIC-FIELD; A SUPERNOVA; TI-44; EJECTA; SHELL; CONSTRAINTS AB We present deep (>2.4 Ms) observations of the Cassiopeia A supernova remnant with NuSTAR, which operates in the 3-79 keV bandpass and is the first instrument capable of spatially resolving the remnant above 15 keV. We find that the emission is not entirely dominated by the forward shock nor by a smooth "bright ring" at the reverse shock. Instead we find that the >15 keV emission is dominated by knots near the center of the remnant and dimmer filaments near the remnant's outer rim. These regions are fit with unbroken power laws in the 15-50 keV bandpass, though the central knots have a steeper (Gamma similar to-3.35) spectrum than the outer filaments (Gamma similar to-3.06). We argue this difference implies that the central knots are located in the 3-D interior of the remnant rather than at the outer rim of the remnant and seen in the center due to projection effects. The morphology of >15 keV emission does not follow that of the radio emission nor that of the low energy (<12 keV) X-rays, leaving the origin of the >15 keV emission an open mystery. Even at the forward shock front we find less steepening of the spectrum than expected from an exponentially cut off electron distribution with a single cutoff energy. Finally, we find that the GeV emission is not associated with the bright features in the NuSTAR band while the TeV emission may be, suggesting that both hadronic and leptonic emission mechanisms may be at work. C1 [Grefenstette, Brian W.; Harrison, Fiona A.; Madsen, Kristin K.; Miyasaka, Hiromasa; Forster, Karl] CALTECH, Cahill Ctr Astrophys, Pasadena, CA 91125 USA. [Reynolds, Stephen P.] N Carolina State Univ, Dept Phys, Raleigh, NC 27695 USA. [Humensky, T. Brian] Columbia Univ, Dept Phys, New York, NY 10027 USA. [Boggs, Steven E.; Zoglauer, Andreas; Craig, William W.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Fryer, Chris L.] Los Alamos Natl Lab, CCS 2, Los Alamos, NM 87545 USA. [DeLaney, Tracey; Zhang, William W.] West Virginia Wesleyan Coll, Phys & Engn Dept, Buckhannon, WV 26201 USA. [Wik, Daniel R.] NASA, Goddard Space Flight Ctr, Astrophys Sci Div, Greenbelt, MD 20771 USA. [Wik, Daniel R.] Johns Hopkins Univ, Dept Phys & Astron, Baltimore, MD 21218 USA. [Kitaguchi, Takao] RIKEN, Wako, Saitama 3510198, Japan. [Lopez, Laura] MIT, Kavli Inst Astrophys & Space Res, Cambridge, MA 02139 USA. [Nynka, Melania; Hailey, Charles J.] Columbia Univ, Columbia Astrophys Lab, New York, NY 10027 USA. [Christensen, Finn E.] Tech Univ Denmark, Natl Space Inst, DTU Space, DK-2800 Lyngby, Denmark. [Stern, Daniel] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. RP Grefenstette, BW (reprint author), CALTECH, Cahill Ctr Astrophys, 1216 E Calif Blvd, Pasadena, CA 91125 USA. EM bwgref@srl.caltech.edu RI Boggs, Steven/E-4170-2015; OI Boggs, Steven/0000-0001-9567-4224; Madsen, Kristin/0000-0003-1252-4891 FU NASA [NNG08FD60C]; NASA FX B.G. thanks Una Hwang for the Chandra 4-6 keV band image. This work was supported under NASA contract NNG08FD60C and made use of data from the NuSTAR mission, a project led by the California Institute of Technology, managed by the Jet Propulsion Laboratory, and funded by NASA. We thank the NuSTAR Operations, Software, and Calibration teams for support with the execution and analysis of these observations. This research has made use of the NuSTAR Data Analysis Software (NuSTARDAS), jointly developed by the ASI Science Data Center (ASDC, Italy) and the California Institute of Technology (USA). NR 51 TC 5 Z9 5 U1 0 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAR 20 PY 2015 VL 802 IS 1 AR 15 DI 10.1088/0004-637X/802/1/15 PG 11 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CE4XW UT WOS:000351834700015 ER PT J AU Jee, MJ Stroe, A Dawson, W Wittman, D Hoekstra, H Bruggen, M Rottgering, H Sobral, D van Weeren, RJ AF Jee, M. James Stroe, Andra Dawson, William Wittman, David Hoekstra, Henk Brueggen, Marcus Rottgering, Huub Sobral, David van Weeren, Reinout J. TI MC2: CONSTRAINING THE DARK MATTER DISTRIBUTION OF THE VIOLENT MERGING GALAXY CLUSTER CIZA J2242.8+5301 BY PIERCING THROUGH THE MILKY WAY SO ASTROPHYSICAL JOURNAL LA English DT Article DE gravitational lensing: weak ID HUBBLE-SPACE-TELESCOPE; DIGITAL SKY SURVEY; ACT-CL J0102-4915; RADIO TELESCOPE; EL GORDO; DISCOVERY; COSMOLOGY; MERGERS; CORE; SUBSTRUCTURE AB The galaxy cluster CIZA J2242.8+5301 at z = 0.19 is a merging system with a prominent (similar to 2Mpc long) radio relic, which together with the morphology of the X-ray emission provides strong evidence for a violent collision along the north-south axis. We present our constraints on the dark matter distribution of this unusual system using Subaru and Canada-France-Hawaii Telescope imaging data. Measuring a high signal-to-noise ratio lensing signal from this cluster is potentially a challenging task because of its proximity to the Milky Way plane (vertical bar b vertical bar similar to 5 degrees). We overcome this challenge with careful observation planning and systematics control, which enables us to successfully map the dark matter distribution of the cluster with high fidelity. The resulting mass map shows that the mass distribution of CIZA J2242.8+5301 is highly elongated along the north-south merger axis inferred from the orientation of the radio relics. Based on our mass reconstruction, we identify two sub-clusters, which coincide with the cluster galaxy distributions. We determine their masses using Markov Chain Monte Carlo analysis by simultaneously fitting two Navarro-Frenk-White halos without fixing their centroids. The resulting masses of the northern and southern systems are M-200 = 11.0(-3.2)(+3.7) x 10(14)M(circle dot) and 9.8(-2.5)(+3.8) x 10(14)M(circle dot), respectively, indicating that we are witnessing a post-collision of two giant systems of nearly equal mass. When the mass and galaxy centroids are compared in detail, we detect similar to 1' (similar to 190 kpc) offsets in both northern and southern sub-clusters. After investigating the statistical significance of the offsets by bootstrapping both mass and galaxy centroids, we find that the galaxy luminosity-mass offset for the northern clump is statistically significant at the greater than or similar to 2 sigma level whereas the detection is only marginal for the southern sub-cluster in part because of a relatively large mass centroid error. We conclude that it is yet premature to uniquely attribute the galaxy-mass misalignment to self-interaction of dark matter and discuss caveats. C1 [Jee, M. James; Wittman, David] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. [Stroe, Andra; Hoekstra, Henk; Rottgering, Huub; Sobral, David] Leiden Univ, Leiden Observ, NL-2300 RA Leiden, Netherlands. [Dawson, William] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Brueggen, Marcus] Hamburger Sternwarte, D-21029 Hamburg, Germany. [Sobral, David] Univ Lisbon, Inst Astrofis & Ciencias Espaco, OAL, PT-1349018 Lisbon, Portugal. [Sobral, David] Univ Lisbon, Ctr Astron & Astrofis, Observ Astron Lisboa, P-1349018 Lisbon, Portugal. [van Weeren, Reinout J.] Harvard Smithsonian Ctr Astrophys, Cambridge, MA 02138 USA. RP Jee, MJ (reprint author), Univ Calif Davis, Dept Phys, One Shields Ave, Davis, CA 95616 USA. RI Sobral, David/C-7919-2014; OI Sobral, David/0000-0001-8823-4845; Wittman, David/0000-0002-0813-5888; van Weeren, Reinout/0000-0002-0587-1660 FU U.S. DOE by LLNL [DE-AC52-07NA27344]; NWO; Deutsche Forschungsgemeinschaft [SFB 676]; Netherlands Organisation for Scientific research (NWO) through a Veni fellowship; FCT through a FCT Investigator Starting Grant and Start-up Grant [IF/01154/2012/CP0189/CT0010]; FCT [PEst-OE/FIS/UI2751/2014]; NASA through the Einstein Postdoctoral awarded by the Chandra X-Ray Center [PF2-130104]; Smithsonian Astrophysical Observatory for NASA [NAS8-03060]; [HST-GO-13343.01-A] FX We thank the Merging Cluster Collaboration for useful discussions and comments. M.J.J., D.W., and W.D. acknowledge support from HST-GO-13343.01-A. Part of this work was performed under the auspices of the U.S. DOE by LLNL under Contract DE-AC52-07NA27344. A.S. acknowledges financial support from NWO. M.B. acknowledges funding from the Deutsche Forschungsgemeinschaft under SFB 676. D.S. acknowledges financial support from the Netherlands Organisation for Scientific research (NWO) through a Veni fellowship, from FCT through a FCT Investigator Starting Grant and Start-up Grant (IF/01154/2012/CP0189/CT0010) and from FCT grant PEst-OE/FIS/UI2751/2014. R.W. is supported by NASA through the Einstein Postdoctoral grant number PF2-130104 awarded by the Chandra X-Ray Center, which is operated by the Smithsonian Astrophysical Observatory for NASA under contract NAS8-03060. NR 54 TC 8 Z9 8 U1 2 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAR 20 PY 2015 VL 802 IS 1 AR 46 DI 10.1088/0004-637X/802/1/46 PG 14 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CE4XW UT WOS:000351834700046 ER PT J AU Lin, HW McDonald, M Benson, B Miller, E AF Lin, Henry W. McDonald, Michael Benson, Bradford Miller, Eric TI COOL CORE BIAS IN SUNYAEV-ZEL'DOVICH GALAXY CLUSTER SURVEYS SO ASTROPHYSICAL JOURNAL LA English DT Article DE cosmology: observations; galaxies: clusters: general; galaxies: clusters: intracluster medium ID SOUTH-POLE TELESCOPE; SUPERMASSIVE BLACK-HOLE; X-RAY CAVITIES; NONTHERMAL PRESSURE; SCALING RELATIONS; RADIO-SOURCES; SAMPLE; MASS; GAS; NEARBY AB Sunyaev-Zel'dovich (SZ) surveys find massive clusters of galaxies by measuring the inverse Compton scattering of cosmic microwave background off of intra-cluster gas. The cluster selection function from such surveys is expected to be nearly independent of redshift and cluster astrophysics. In this work, we estimate the effect on the observed SZ signal of centrally peaked gas density profiles (cool cores) and radio emission from the brightest cluster galaxy by creating mock observations of a sample of clusters that span the observed range of classical cooling rates and radio luminosities. For each cluster, we make simulated SZ observations by the South Pole Telescope and characterize the cluster selection function, but note that our results are broadly applicable to other SZ surveys. We find that the inclusion of a cool core can cause a change in the measured SPT significance of a cluster between 0.01 and 10% at z > 0.3, increasing with cuspiness of the cool core and angular size on the sky of the cluster (i.e., decreasing redshift, increasing mass). We provide quantitative estimates of the bias in the SZ signal as a function of a gas density cuspiness parameter, redshift, mass, and the 1.4 GHz radio luminosity of the central active galactic nuclei. Based on this work, we estimate that, for the Phoenix cluster (one of the strongest cool cores known), the presence of a cool core is biasing the SZ significance high by similar to 6%. The ubiquity of radio galaxies at the centers of cool core clusters will offset the cool core bias to varying degrees. C1 [Lin, Henry W.] Harvard Univ, Cambridge, MA 02138 USA. [McDonald, Michael; Miller, Eric] MIT, Kavli Inst Astrophys & Space Res, Cambridge, MA 02139 USA. [Benson, Bradford] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Benson, Bradford] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Benson, Bradford] Univ Chicago, Dept Astron & Astrophys, Chicago, IL 60637 USA. RP Lin, HW (reprint author), Harvard Univ, Cambridge, MA 02138 USA. EM henrylin@college.harvard.edu OI Lin, Henry/0000-0003-2767-6142 NR 58 TC 4 Z9 4 U1 0 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAR 20 PY 2015 VL 802 IS 1 AR 34 DI 10.1088/0004-637X/802/1/34 PG 8 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CE4XW UT WOS:000351834700034 ER PT J AU Medin, Z Cumming, A AF Medin, Zach Cumming, Andrew TI TIME-DEPENDENT, COMPOSITIONALLY DRIVEN CONVECTION IN THE OCEANS OF ACCRETING NEUTRON STARS SO ASTROPHYSICAL JOURNAL LA English DT Article DE dense matter; stars: neutron; X-rays: binaries ID X-RAY TRANSIENT; PLANETARY MAGNETIC-FIELDS; COOLING LIGHT CURVES; BINARY MXB 1659-29; SUPERBURST IGNITION; CHANDRA OBSERVATION; XTE J1701-462; EXO 0748-676; CRUST; QUIESCENCE AB We discuss the effect of convection driven by chemical separation at the ocean-crust boundary of accreting neutron stars. We extend the steady-state results of Medin & Cumming to transient accretors, by considering the time-dependent cases of heating during accretion outbursts and cooling during quiescence. During accretion outbursts, inward heat transport has only a small effect on the temperature profile in the outer layers until the ocean is strongly enriched in light elements, a process that takes hundreds of years to complete. During quiescence, however, inward heat transport rapidly cools the outer layers of the ocean while keeping the inner layers hot. We find that this leads to a sharp drop in surface emission at around a week followed by a gradual recovery as cooling becomes dominated by the crust. Such a dip should be observable in the light curves of these neutron star transients, if enough data is taken at a few days to a month after the end of accretion. If such a dip is definitively observed, it will provide strong constraints on the chemical composition of the ocean and outer crust. C1 [Medin, Zach] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Cumming, Andrew] McGill Univ, Dept Phys, Montreal, PQ H3A 2T8, Canada. RP Medin, Z (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM zmedin@lanl.gov; cumming@physics.mcgill.ca FU LANL Director's Postdoctoral Fellowship; NSERC; Centre de Recherche en Astrophysique du Quebec (CRAQ); Associate of the CIFAR Cosmology and Gravity program; National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory [AC52-06NA25396] FX We thank Chuck Horowitz, Nathalie Degenaar, and Chris Fontes for useful discussions. Z.M. was supported by a LANL Director's Postdoctoral Fellowship. A.C. is supported by an NSERC Discovery grant, and is a member of the Centre de Recherche en Astrophysique du Quebec (CRAQ) and an Associate of the CIFAR Cosmology and Gravity program. This research was carried out in part under the auspices of the National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory and supported by Contract No. DE-AC52-06NA25396. NR 56 TC 4 Z9 4 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAR 20 PY 2015 VL 802 IS 1 AR 29 DI 10.1088/0004-637X/802/1/29 PG 18 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CE4XW UT WOS:000351834700029 ER PT J AU Rigault, M Aldering, G Kowalski, M Copin, Y Antilogus, P Aragon, C Bailey, S Baltay, C Baugh, D Bongard, S Boone, K Buton, C Chen, J Chotard, N Fakhouri, HK Feindt, U Fagrelius, P Fleury, M Fouchez, D Gangler, E Hayden, B Kim, AG Leget, PF Lombardo, S Nordin, J Pain, R Pecontal, E Pereira, R Perlmutter, S Rabinowitz, D Runge, K Rubin, D Saunders, C Smadja, G Sofiatti, C Suzuki, N Tao, C Weaver, BA AF Rigault, M. Aldering, G. Kowalski, M. Copin, Y. Antilogus, P. Aragon, C. Bailey, S. Baltay, C. Baugh, D. Bongard, S. Boone, K. Buton, C. Chen, J. Chotard, N. Fakhouri, H. K. Feindt, U. Fagrelius, P. Fleury, M. Fouchez, D. Gangler, E. Hayden, B. Kim, A. G. Leget, P. -F. Lombardo, S. Nordin, J. Pain, R. Pecontal, E. Pereira, R. Perlmutter, S. Rabinowitz, D. Runge, K. Rubin, D. Saunders, C. Smadja, G. Sofiatti, C. Suzuki, N. Tao, C. Weaver, B. A. TI CONFIRMATION OF A STAR FORMATION BIAS IN TYPE Ia SUPERNOVA DISTANCES AND ITS EFFECT ON THE MEASUREMENT OF THE HUBBLE CONSTANT SO ASTROPHYSICAL JOURNAL LA English DT Article DE cosmology: observations; distance scale; galaxies: distances and redshifts; supernovae: general; ultraviolet: galaxies ID HOST-GALAXY PROPERTIES; DIFFUSE H-ALPHA; FORMATION RATES; LIGHT CURVES; SPACE-TELESCOPE; FAR-ULTRAVIOLET; COSMOLOGICAL PARAMETERS; ANTENNAE GALAXIES; DUST ATTENUATION; INFRARED TRACERS AB Previously we used the Nearby Supernova Factory sample to show that Type Ia supernovae (SNe Ia) having locally star-forming environments are dimmer than SNe Ia having locally passive environments. Here we use the Constitution sample together with host galaxy data from GALEX to independently confirm that result. The effect is seen using both the SALT2 and MLCS2k2 lightcurve fitting and standardization methods, with brightness differences of 0.094 +/- 0.037 mag for SALT2 and 0.155 +/- 0.041 mag for MLCS2k2 with R-V = 2.5. When combined with our previous measurement the effect is 0.094 +/- 0.025 mag for SALT2. If the ratio of these local SN Ia environments changes with redshift or sample selection, this can lead to a bias in cosmological measurements. We explore this issue further, using as an example the direct measurement of H-0. GALEX observations show that the SNe Ia having standardized absolute magnitudes calibrated via the Cepheid period-luminosity relation using the Hubble Space Telescope originate in predominately star-forming environments, whereas only similar to 50% of the Hubble-flow comparison sample have locally star-forming environments. As a consequence, the H-0 measurement using SNe Ia is currently overestimated. Correcting for this bias, we find a value of H-0(corr) = 70.6 +/- 2.6 km s(-1) Mpc(-1) when using the LMC distance, Milky Way parallaxes, and the NGC 4258 megamaser as the Cepheid zero point, and 68.8 +/- 3.3 km s(-1) Mpc(-1) when only using NGC 4258. Our correction brings the direct measurement of H-0 within similar to 1 sigma of recent indirect measurements based on the cosmic microwave background power spectrum. C1 [Rigault, M.; Kowalski, M.; Feindt, U.; Lombardo, S.; Nordin, J.] Humboldt Univ, Inst Phys, D-12489 Berlin, Germany. [Aldering, G.; Aragon, C.; Bailey, S.; Boone, K.; Fakhouri, H. K.; Fagrelius, P.; Hayden, B.; Kim, A. G.; Nordin, J.; Perlmutter, S.; Runge, K.; Rubin, D.; Saunders, C.; Sofiatti, C.; Suzuki, N.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Kowalski, M.] DESY, D-15735 Zeuthen, Germany. [Copin, Y.; Chotard, N.; Pereira, R.; Smadja, G.] Univ Lyon 1, Inst Phys Nucl Lyon, IN2P3, CNRS, F-69622 Villeurbanne, France. [Antilogus, P.; Bongard, S.; Fleury, M.; Pain, R.] Univ Paris Diderot Paris, Univ Paris 06, Lab Phys Nucl & Hautes Energies, CNRS,IN2P3, F-75005 Paris, France. [Aragon, C.] Univ Washington, Coll Engn, Seattle, WA 98195 USA. [Baltay, C.; Rabinowitz, D.; Tao, C.] Yale Univ, Dept Phys, New Haven, CT 06250 USA. [Baugh, D.; Chen, J.] Tsinghua Univ, Tsinghua Ctr Astrophys, Beijing 100084, Peoples R China. [Boone, K.; Fagrelius, P.; Perlmutter, S.; Sofiatti, C.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Feindt, U.] Univ Bonn, Inst Phys, D-53115 Bonn, Germany. [Fouchez, D.; Tao, C.] Aix Marseille Univ, Ctr Phys Particules Marseille, IN2P3, CNRS, F-13288 Marseille 09, France. [Gangler, E.; Leget, P. -F.] Aix Marseille Univ, Ctr Phys Particules Marseille, IN2P3, CNRS, F-13288 Marseille 09, France. [Pecontal, E.] Univ Lyon 1, Ctr Rech Astron Lyon, F-69561 St Genis Laval, France. [Rubin, D.] Florida State Univ, Dept Phys, Tallahassee, FL 32306 USA. [Suzuki, N.; Weaver, B. A.] NYU, Ctr Cosmol & Particle Phys, New York, NY 10003 USA. RP Rigault, M (reprint author), Humboldt Univ, Inst Phys, Newtonstr 15, D-12489 Berlin, Germany. RI Copin, Yannick/B-4928-2015; OI Copin, Yannick/0000-0002-5317-7518; Boone, Kyle/0000-0002-5828-6211 FU NASA [NAS5-98034, NAS5-26555]; Office of Science, Office of High Energy Physics, of the U.S. Department of Energy [DE-AC02-05CH11231]; DFG [TRR33]; CNRS/IN2P3; CNRS/INSU; PNC; Tsinghua University [985]; NSFC [11173017]; LABEX ILP; French state funds [ANR-11-IDEX-0004-02]; LABEX Lyon Institute of Origins of the Universite de Lyon of the French government [ANR-10-LABX-0066, ANR-11-IDEX-0007]; NASA Office of Space Science [NNX13AC07G] FX We thank Jake Simones, Evan Skillman, Adam Riess, Robert Kirshner, and Saurahb Jha for useful discussions. This work is based on observations made with the NASA Galaxy Evolution Explorer. GALEX is operated for NASA by the California Institute of Technology under NASA contract NAS5-98034. This work was supported in part by the Director, Office of Science, Office of High Energy Physics, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231; in Germany by the DFG through TRR33 "The Dark Universe"; in France by support from CNRS/IN2P3, CNRS/INSU, and PNC; and in China from Tsinghua University 985 grant and NSFC grant No. 11173017. LPNHE acknowledges support from LABEX ILP, supported by French state funds managed by the ANR within the Investissements d'Avenir programme under reference ANR-11-IDEX-0004-02. NC is grateful to the LABEX Lyon Institute of Origins (ANR-10-LABX-0066) of the Universite de Lyon for its financial support within the program "Investissements d'Avenir" (ANR-11-IDEX-0007) of the French government operated by the National Research Agency (ANR). This research has made use of the NASA/IPAC Extragalactic Database (NED), which is operated by the Jet Propulsion Laboratory, California Institute of Technology, under contract with the National Aeronautics and Space Administration. Some of the data presented in this paper were obtained from the Mikulski Archive for Space Telescopes (MAST). STScI is operated by the Association of Universities for Research in Astronomy, Inc., under NASA contract NAS5-26555. Support for MAST for non-HST data is provided by the NASA Office of Space Science via grant NNX13AC07G and by other grants and contracts. NR 93 TC 26 Z9 26 U1 0 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAR 20 PY 2015 VL 802 IS 1 AR 20 DI 10.1088/0004-637X/802/1/20 PG 18 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CE4XW UT WOS:000351834700020 ER PT J AU Staquicini, FI Qian, MD Salameh, A Dobroff, AS Edwards, JK Cimino, DF Moeller, BJ Kelly, P Nunez, MI Tang, XM Liu, DD Lee, JJ Hong, WK Ferrara, F Bradbury, ARM Lobb, RR Edelman, MJ Sidman, RL Wistuba, II Arap, W Pasqualini, R AF Staquicini, Fernanda I. Qian, Ming D. Salameh, Ahmad Dobroff, Andrey S. Edwards, Julianna K. Cimino, Daniel F. Moeller, Benjamin J. Kelly, Patrick Nunez, Maria I. Tang, Ximing Liu, Diane D. Lee, J. Jack Hong, Waun Ki Ferrara, Fortunato Bradbury, Andrew R. M. Lobb, Roy R. Edelman, Martin J. Sidman, Richard L. Wistuba, Ignacio I. Arap, Wadih Pasqualini, Renata TI Receptor Tyrosine Kinase EphA5 Is a Functional Molecular Target in Human Lung Cancer SO JOURNAL OF BIOLOGICAL CHEMISTRY LA English DT Article DE Cell Cycle; DNA Damage; DNA Damage Response; DNA Repair; Monoclonal Antibody; Receptor Tyrosine Kinase; Ionizing Radiation ID DEPENDENT PROTEIN-KINASE; GROWTH-FACTOR RECEPTOR; DNA-DAMAGE RESPONSE; ATAXIA-TELANGIECTASIA; IONIZING IRRADIATION; SIGNALING NETWORKS; GENOME INTEGRITY; CELL-CYCLE; ATM; EXPRESSION AB Background: EphA5 is a functional target in lung cancer, the most common cause of tumor-related death in mankind. Results: EphA5 regulates cell cycle checkpoints and DNA damage repair induced by ionizing radiation. Conclusion: EphA5 is a novel regulator of DNA damage repair with clinical implications. Significance: EphA5 may serve as a novel biomarker of radioresistance and a candidate target for therapeutic intervention in human lung cancer. Lung cancer is often refractory to radiotherapy, but molecular mechanisms of tumor resistance remain poorly defined. Here we show that the receptor tyrosine kinase EphA5 is specifically overexpressed in lung cancer and is involved in regulating cellular responses to genotoxic insult. In the absence of EphA5, lung cancer cells displayed a defective G(1)/S cell cycle checkpoint, were unable to resolve DNA damage, and became radiosensitive. Upon irradiation, EphA5 was transported into the nucleus where it interacted with activated ATM (ataxia-telangiectasia mutated) at sites of DNA repair. Finally, we demonstrate that a new monoclonal antibody against human EphA5 sensitized lung cancer cells and human lung cancer xenografts to radiotherapy and significantly prolonged survival, thus suggesting the likelihood of translational applications. C1 [Staquicini, Fernanda I.; Dobroff, Andrey S.; Cimino, Daniel F.; Ferrara, Fortunato; Arap, Wadih; Pasqualini, Renata] Univ New Mexico, Ctr Canc, Albuquerque, NM 87131 USA. [Staquicini, Fernanda I.; Dobroff, Andrey S.; Cimino, Daniel F.; Ferrara, Fortunato; Pasqualini, Renata] Univ New Mexico, Sch Med, Dept Internal Med, Div Mol Med, Albuquerque, NM 87131 USA. Univ New Mexico, Sch Med, Dept Internal Med, Div Hematol Med Oncol, Albuquerque, NM 87131 USA. [Qian, Ming D.; Salameh, Ahmad; Edwards, Julianna K.; Moeller, Benjamin J.; Kelly, Patrick] Univ Texas MD Anderson Canc Ctr, David H Koch Ctr, Dept Genitourinary Med Oncol, Houston, TX 77030 USA. [Moeller, Benjamin J.; Kelly, Patrick] Univ Texas MD Anderson Canc Ctr, David H Koch Ctr, Dept Radiat Oncol, Houston, TX 77030 USA. [Nunez, Maria I.; Tang, Ximing; Wistuba, Ignacio I.] Univ Texas MD Anderson Canc Ctr, David H Koch Ctr, Dept Translat Mol Pathol, Houston, TX 77030 USA. [Liu, Diane D.; Lee, J. Jack] Univ Texas MD Anderson Canc Ctr, David H Koch Ctr, Dept Biostat, Houston, TX 77030 USA. [Hong, Waun Ki] Univ Texas MD Anderson Canc Ctr, David H Koch Ctr, Dept Thorac Head & Neck Med Oncol, Houston, TX 77030 USA. [Bradbury, Andrew R. M.] Los Alamos Natl Lab, Biosci Div, Los Alamos, NM 87545 USA. [Lobb, Roy R.; Edelman, Martin J.] Arrowhead Res Corp, Alvos Therapeut, Pasadena, CA 91101 USA. Univ Maryland, Sch Med, Baltimore, MD 21201 USA. [Sidman, Richard L.] Harvard Univ, Beth Israel Deaconess Med Ctr, Sch Med, Dept Neurol, Boston, MA 02215 USA. RP Arap, W (reprint author), Univ New Mexico, Ctr Canc, Albuquerque, NM 87131 USA. EM warap@salud.unm.edu; rpasqual@salud.unm.edu RI Dobroff, Andrey/A-9814-2016; OI Dobroff, Andrey/0000-0003-2162-9951; Bradbury, Andrew/0000-0002-5567-8172 FU National Institutes of Health; National Cancer Institute; Department of Defense; Specialized Program of Research Excellence in Lung Cancer FX This work was supported, in whole or in part, by National Institutes of Health Grants (to R. P. and W. A.). This work was also supported by funds from the National Cancer Institute (to R. P., W. A., and I. I. W.), the Department of Defense (to R. P., W. A., I. I. W., and W. K. H.), and the Specialized Program of Research Excellence in Lung Cancer (to I. I. W.). The University of Texas M. D. Anderson Cancer Center and some of its researchers at the time (W. A. and R. P.) had equity positions in Alvos Therapeutics (Arrowhead Research Corporation, Pasadena, CA), which was subjected to certain restrictions under university policy; the University manages and monitors the terms of these arrangements in accordance with its conflict-of-interest policy. F. I. S., W. A., and R. P. are coinventors of issued patents filed by Alvos Therapeutics that cover the mAb 11C12 and are entitled to royalties that could result from commercial success of the drug. NR 40 TC 7 Z9 7 U1 1 U2 5 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 0021-9258 EI 1083-351X J9 J BIOL CHEM JI J. Biol. Chem. PD MAR 20 PY 2015 VL 290 IS 12 BP 7345 EP 7359 DI 10.1074/jbc.M114.630525 PG 15 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CE2AC UT WOS:000351613600003 PM 25623065 ER PT J AU Allan, CM Awad, AM Johnson, JS Shirasaki, DI Wang, C Blaby-Haas, CE Merchant, SS Loo, JA Clarke, CF AF Allan, Christopher M. Awad, Agape M. Johnson, Jarrett S. Shirasaki, Dyna I. Wang, Charles Blaby-Haas, Crysten E. Merchant, Sabeeha S. Loo, Joseph A. Clarke, Catherine F. TI Identification of Coq11, a New Coenzyme Q Biosynthetic Protein in the CoQ-Synthome in Saccharomyces cerevisiae SO JOURNAL OF BIOLOGICAL CHEMISTRY LA English DT Article DE Mass Spectrometry (MS); Mitochondrial Metabolism; Protein Complex; Proteomics; Saccharomyces cerevisiae; Ubiquinone; Yeast; Q Biosynthetic Intermediates; Coenzyme Q; Immunoprecipitation ID PARA-AMINOBENZOIC ACID; MITOCHONDRIAL FERREDOXIN; C-METHYLTRANSFERASE; YEAST MITOCHONDRIA; BINDING-PROTEIN; ACETOHYDROXYACID SYNTHASE; UBIQUINONE BIOSYNTHESIS; ACETOLACTATE SYNTHASE; ADRENODOXIN REDUCTASE; REGULATORY SUBUNIT AB Background: Yeast synthesizes coenzyme Q via a macromolecular protein complex. Results: The Q biosynthetic complex includes Coq8 and the uncharacterized protein YLR290C; the ylr290c mutant exhibits impaired Q synthesis. Conclusion: YLR290C (Coq11) is a novel protein required for efficient yeast Q biosynthesis. Significance: Discovery and characterization of yeast Coq biosynthetic proteins leads to an improved understanding of coenzyme Q biosynthesis and regulation. Coenzyme Q (Q or ubiquinone) is a redox active lipid composed of a fully substituted benzoquinone ring and a polyisoprenoid tail and is required for mitochondrial electron transport. In the yeast Saccharomyces cerevisiae, Q is synthesized by the products of 11 known genes, COQ1-COQ9, YAH1, and ARH1. The function of some of the Coq proteins remains unknown, and several steps in the Q biosynthetic pathway are not fully characterized. Several of the Coq proteins are associated in a macromolecular complex on the matrix face of the inner mitochondrial membrane, and this complex is required for efficient Q synthesis. Here, we further characterize this complex via immunoblotting and proteomic analysis of tandem affinity-purified tagged Coq proteins. We show that Coq8, a putative kinase required for the stability of the Q biosynthetic complex, is associated with a Coq6-containing complex. Additionally Q(6) and late stage Q biosynthetic intermediates were also found to co-purify with the complex. A mitochondrial protein of unknown function, encoded by the YLR290C open reading frame, is also identified as a constituent of the complex and is shown to be required for efficient de novo Q biosynthesis. Given its effect on Q synthesis and its association with the biosynthetic complex, we propose that the open reading frame YLR290C be designated COQ11. C1 [Allan, Christopher M.; Awad, Agape M.; Johnson, Jarrett S.; Shirasaki, Dyna I.; Wang, Charles; Blaby-Haas, Crysten E.; Merchant, Sabeeha S.; Loo, Joseph A.; Clarke, Catherine F.] Univ Calif Los Angeles, Dept Chem & Biochem, Los Angeles, CA 90095 USA. [Allan, Christopher M.; Awad, Agape M.; Johnson, Jarrett S.; Shirasaki, Dyna I.; Wang, Charles; Blaby-Haas, Crysten E.; Merchant, Sabeeha S.; Loo, Joseph A.; Clarke, Catherine F.] Univ Calif Los Angeles, Inst Mol Biol, Los Angeles, CA 90095 USA. [Loo, Joseph A.] Univ Calif Los Angeles, Dept Biol Chem, Los Angeles, CA 90095 USA. [Merchant, Sabeeha S.; Loo, Joseph A.] Univ Calif Los Angeles, US DOE, Inst Genom & Prote, Los Angeles, CA 90095 USA. RP Clarke, CF (reprint author), Univ Calif Los Angeles, Dept Chem & Biochem, 607 Charles E Young Dr E,Box 156905, Los Angeles, CA 90095 USA. EM cathy@chem.ucla.edu OI Blaby, Crysten/0000-0002-1583-1291 FU National Institutes of Health [S10RR024605, R01GM103479]; National Science Foundation [MCB-1330803]; Kirschstein National Research Service Award NIH [GM100753]; Office of Science (Biological and Environmental Research), U.S. Department of Energy [DE-FC02-02ER63421] FX This work was supported, in whole or in part, by National Institutes of Health Grants S10RR024605 and R01GM103479 (to J. A. L.). This work was also supported by National Science Foundation Grant MCB-1330803 (to C. F. C.), Kirschstein National Research Service Award NIH GM100753 (to C. E. B.-H.), and Grant DE-FC02-02ER63421 from the Office of Science (Biological and Environmental Research), U.S. Department of Energy. NR 90 TC 10 Z9 10 U1 0 U2 9 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 0021-9258 EI 1083-351X J9 J BIOL CHEM JI J. Biol. Chem. PD MAR 20 PY 2015 VL 290 IS 12 BP 7517 EP 7534 DI 10.1074/jbc.M114.633131 PG 18 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CE2AC UT WOS:000351613600019 PM 25631044 ER PT J AU Kudalkar, SN Nikas, SP Kingsley, PJ Xu, S Galligan, JJ Rouzer, CA Banerjee, S Ji, LP Eno, MR Makriyannis, A Marnett, LJ AF Kudalkar, Shalley N. Nikas, Spyros P. Kingsley, Philip J. Xu, Shu Galligan, James J. Rouzer, Carol A. Banerjee, Surajit Ji, Lipin Eno, Marsha R. Makriyannis, Alexandros Marnett, Lawrence J. TI 13-Methylarachidonic Acid Is a Positive Allosteric Modulator of Endocannabinoid Oxygenation by Cyclooxygenase SO JOURNAL OF BIOLOGICAL CHEMISTRY LA English DT Article DE Allosteric Regulation; Cyclooxygenase (COX); Endocannabinoid; Enzyme Kinetics; Site-directed Mutagenesis ID COX-2 OXIDATIVE METABOLITE; PROSTAGLANDIN-H SYNTHASE; SYNAPTIC-TRANSMISSION; SEQUENCE HOMODIMER; ARACHIDONIC-ACID; STRUCTURAL BASIS; GLYCEROL ESTER; FATTY-ACIDS; CROSS-TALK; INHIBITION AB Background: The structurally identical monomers of cyclooxygenase-2 act as distinct catalytic and allosteric subunits. Results: 13-Methylarachidonic acid strongly potentiates cyclooxygenase-2-mediated endocannabinoid oxygenation without affecting arachidonic acid oxygenation. Conclusion: 13-Methylarachidonic acid is a substrate-selective allosteric potentiator of cyclooxygenase-2-mediated endocannabinoid oxygenation. Significance: 13-Methylarachidonic acid is a valuable tool for probing cyclooxygenase-dependent endocannabinoid oxygenation. Cyclooxygenase-2 (COX-2) oxygenates arachidonic acid (AA) and the endocannabinoids 2-arachidonoylglycerol (2-AG) and arachidonylethanolamide to prostaglandins, prostaglandin glyceryl esters, and prostaglandin ethanolamides, respectively. A structural homodimer, COX-2 acts as a conformational heterodimer with a catalytic and an allosteric monomer. Prior studies have demonstrated substrate-selective negative allosteric regulation of 2-AG oxygenation. Here we describe AM-8138 (13(S)-methylarachidonic acid), a substrate-selective allosteric potentiator that augments 2-AG oxygenation by up to 3.5-fold with no effect on AA oxygenation. In the crystal structure of an AM-8138.COX-2 complex, AM-8138 adopts a conformation similar to the unproductive conformation of AA in the substrate binding site. Kinetic analysis suggests that binding of AM-8138 to the allosteric monomer of COX-2 increases 2-AG oxygenation by increasing k(cat) and preventing inhibitory binding of 2-AG. AM-8138 restored the activity of COX-2 mutants that exhibited very poor 2-AG oxygenating activity and increased the activity of COX-1 toward 2-AG. Competition of AM-8138 for the allosteric site prevented the inhibition of COX-2-dependent 2-AG oxygenation by substrate-selective inhibitors and blocked the inhibition of AA or 2-AG oxygenation by nonselective time-dependent inhibitors. AM-8138 selectively enhanced 2-AG oxygenation in intact RAW264.7 macrophage-like cells. Thus, AM-8138 is an important new tool compound for the exploration of allosteric modulation of COX enzymes and their role in endocannabinoid metabolism. C1 [Kudalkar, Shalley N.; Kingsley, Philip J.; Xu, Shu; Galligan, James J.; Rouzer, Carol A.; Marnett, Lawrence J.] Vanderbilt Univ, Sch Med, AB Hancock Jr Mem Lab Canc Res, Nashville, TN 37232 USA. [Kudalkar, Shalley N.; Kingsley, Philip J.; Xu, Shu; Galligan, James J.; Marnett, Lawrence J.] Vanderbilt Univ, Sch Med, Dept Biochem, Nashville, TN 37232 USA. [Marnett, Lawrence J.] Vanderbilt Univ, Sch Med, Dept Chem, Nashville, TN 37232 USA. [Marnett, Lawrence J.] Vanderbilt Univ, Sch Med, Dept Pharmacol, Nashville, TN 37232 USA. [Rouzer, Carol A.; Marnett, Lawrence J.] Vanderbilt Univ, Sch Med, Vanderbilt Inst Chem Biol, Nashville, TN 37232 USA. [Marnett, Lawrence J.] Vanderbilt Univ, Sch Med, Vanderbilt Ctr Mol Toxicol, Nashville, TN 37232 USA. [Marnett, Lawrence J.] Vanderbilt Univ, Sch Med, Vanderbilt Ingram Canc Ctr, Nashville, TN 37232 USA. [Marnett, Lawrence J.] Vanderbilt Univ, Sch Med, Nashville, TN 37232 USA. [Nikas, Spyros P.; Ji, Lipin; Eno, Marsha R.; Makriyannis, Alexandros] Northeastern Univ, Dept Pharmaceut Sci, Boston, MA 02115 USA. [Banerjee, Surajit] Cornell Univ, Dept Chem & Chem Biol, Ithaca, NY 14853 USA. [Banerjee, Surajit] Argonne Natl Lab, Northeastern Collaborat Access Team, Argonne, IL 60439 USA. RP Marnett, LJ (reprint author), Vanderbilt Univ, Sch Med, AB Hancock Jr Mem Lab Canc Res, Nashville, TN 37232 USA. EM larry.marnett@vanderbilt.edu OI Xu, Shu/0000-0002-6876-7991; Banerjee, Surajit/0000-0002-9414-7163 FU National Institutes of Health from the NIGMS [P41 GM103403]; United States Department of Energy [DE-AC02-06CH11357] FX We thank James A. Wepy for valuable input in developing the AM-8138 potentiation scheme. We also thank William N. Beavers for helpful discussions and suggestions. This work is based upon research conducted at the Advanced Photon Source on the Northeastern Collaborative Access Team beamlines, which are supported by National Institutes of Health Grant P41 GM103403 from the NIGMS. Use of the Advanced Photon Source, an Office of Science User Facility operated for the United States Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the United States Department of Energy under Contract DE-AC02-06CH11357. NR 47 TC 8 Z9 8 U1 0 U2 7 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 0021-9258 EI 1083-351X J9 J BIOL CHEM JI J. Biol. Chem. PD MAR 20 PY 2015 VL 290 IS 12 BP 7897 EP 7909 DI 10.1074/jbc.M114.634014 PG 13 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CE2AC UT WOS:000351613600047 PM 25648895 ER PT J AU Prange, MP Campbell, LW Wu, D Gao, F Kerisit, S AF Prange, M. P. Campbell, L. W. Wu, D. Gao, F. Kerisit, S. TI Calculation of energy relaxation rates of fast particles by phonons in crystals SO PHYSICAL REVIEW B LA English DT Article ID SCINTILLATOR NON-PROPORTIONALITY; SLOW ELECTRONS; ALKALI-HALIDES; POLAR CRYSTAL; TRANSPORT; NONPROPORTIONALITY; PSEUDOPOTENTIALS; DETECTORS; BREAKDOWN; DENSITY AB We present ab initio calculations of the temperature-dependent exchange of energy between a classical charged point particle and the phonons of a crystalline material. The phonons, which are computed using density functional perturbation theory (DFPT) methods, interact with the moving particle via the Coulomb interaction between the density induced in the material by phonon excitation and the charge of the classical particle. Energy relaxation rates are computed using time-dependent perturbation theory. The method, which is applicable wherever DFPT is, is illustrated with results for CsI, an important scintillator whose performance is affected by electron thermalization. We discuss the influence of the form assumed for quasiparticle dispersion on theoretical estimates of electron cooling rates. C1 [Prange, M. P.; Wu, D.; Gao, F.; Kerisit, S.] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99354 USA. [Campbell, L. W.] Pacific NW Natl Lab, Natl Secur Directorate, Richland, WA 99354 USA. [Gao, F.] Univ Michigan, Dept Nucl Engn & Radiol Sci, Ann Arbor, MI 48109 USA. RP Prange, MP (reprint author), Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99354 USA. EM micah.prange@pnnl.gov FU National Nuclear Security Administration, Office of Defense Nuclear Non-proliferation Research and Development (DNN R&D), of the US Department of Energy (DOE); US DOE [DE-AC0576RL01830] FX This research was supported by the National Nuclear Security Administration, Office of Defense Nuclear Non-proliferation Research and Development (DNN R&D), of the US Department of Energy (DOE). A portion of the research was performed using PNNL Institutional Computing at Pacific Northwest National Laboratory (PNNL). PNNL is a multiprogram national laboratory operated by Battelle Memorial Institute for the US DOE under Contract No. DE-AC0576RL01830. NR 37 TC 2 Z9 2 U1 4 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAR 20 PY 2015 VL 91 IS 10 AR 104305 DI 10.1103/PhysRevB.91.104305 PG 8 WC Physics, Condensed Matter SC Physics GA CE8FK UT WOS:000352076900003 ER PT J AU Adamczyk, L Adkins, JK Agakishiev, G Aggarwal, MM Ahammed, Z Alekseev, I Alford, J Anson, CD Aparin, A Arkhipkin, D Aschenauer, EC Averichev, GS Banerjee, A Beavis, DR Bellwied, R Bhasin, A Bhati, AK Bhattarai, P Bichsel, H Bielcik, J Bielcikova, J Bland, LC Bordyuzhin, IG Borowski, W Bouchet, J Brandin, AV Brovko, SG Bultmann, S Bunzarov, I Burton, TP Butterworth, J Caines, H Sanchez, MCD Campbell, JM Cebra, D Cendejas, R Cervantes, MC Chaloupka, P Chang, Z Chattopadhyay, S Chen, HF Chen, JH Chen, L Cheng, J Cherney, M Chikanian, A Christie, W Chwastowski, J Codrington, MJM Contin, G Cramer, JG Crawford, HJ Cui, X Das, S Leyva, AD De Silva, LC Debbe, RR Dedovich, TG Deng, J Derevschikov, AA de Souza, RD di Ruzza, B Didenko, L Dilks, C Ding, F Djawotho, P Dong, X Drachenberg, JL Draper, JE Du, CM Dunkelberger, LE Dunlop, JC Efimov, LG Engelage, J Engle, KS Eppley, G Eun, L Evdokimov, O Eyser, O Fatemi, R Fazio, S Fedorisin, J Filip, P Fisyak, Y Flores, CE Gagliardi, CA Gangadharan, DR Garand, D Geurts, F Gibson, A Girard, M Gliske, S Greiner, L Grosnick, D Gunarathne, DS Guo, Y Gupta, A Gupta, S Guryn, W Haag, B Hamed, A Han, LX Haque, R Harris, JW Heppelmann, S Hirsch, A Hoffmann, GW Hofman, DJ Horvat, S Huang, B Huang, HZ Huang, X Huck, P Humanic, TJ Igo, G Jacobs, WW Jang, H Judd, EG Kabana, S Kalinkin, D Kang, K Kauder, K Ke, HW Keane, D Kechechyan, A Kesich, A Khan, ZH Kikola, DP Kisel, I Kisiel, A Koetke, DD Kollegger, T Konzer, J Koralt, I Kosarzewski, LK Kotchenda, L Kraishan, AF Kravtsov, P Krueger, K Kulakov, I Kumar, L Kycia, RA Lamont, MAC Landgraf, JM Landry, KD Lauret, J Lebedev, A Lednicky, R Lee, JH Li, C Li, W Li, X Li, X Li, Y Li, ZM Lisa, MA Liu, F Ljubicic, T Llope, WJ Lomnitz, M Longacre, RS Luo, X Ma, GL Ma, YG Mahapatra, DP Majka, R Margetis, S Markert, C Masui, H Matis, HS McDonald, D McShane, TS Minaev, NG Mioduszewski, S Mohanty, B Mondal, MM Morozov, DA Mustafa, MK Nandi, BK Nasim, M Nayak, TK Nelson, JM Nigmatkulov, G Nogach, LV Noh, SY Novak, J Nurushev, SB Odyniec, G Ogawa, A Oh, K Ohlson, A Okorokov, V Oldag, EW Olvitt, DL Page, BS Pan, YX Pandit, Y Panebratsev, Y Pawlak, T Pawlik, B Pei, H Perkins, C Pile, P Planinic, M Pluta, J Poljak, N Poniatowska, K Porter, J Poskanzer, AM Pruthi, NK Przybycien, M Putschke, J Qiu, H Quintero, A Ramachandran, S Raniwala, R Raniwala, S Ray, RL Riley, CK Ritter, HG Roberts, JB Rogachevskiy, OV Romero, JL Ross, JF Roy, A Ruan, L Rusnak, J Rusnakova, O Sahoo, NR Sahu, PK Sakrejda, I Salur, S Sandacz, A Sandweiss, J Sangaline, E Sarkar, A Schambach, J Scharenberg, RP Schmah, AM Schmidke, WB Schmitz, N Seger, J Seyboth, P Shah, N Shahaliev, E Shanmuganathan, PV Shao, M Sharma, B Shen, WQ Shi, SS Shou, QY Sichtermann, EP Simko, M Skoby, MJ Smirnov, D Smirnov, N Solanki, D Sorensen, P Spinka, HM Srivastava, B Stanislaus, TDS Stevens, JR Stock, R Strikhanov, M Stringfellow, B Sumbera, M Sun, X Sun, XM Sun, Y Sun, Z Surrow, B Svirida, DN Symons, TJM Szelezniak, MA Takahashi, J Tang, AH Tang, Z Tarnowsky, T Thomas, JH Timmins, AR Tlusty, D Tokarev, M Trentalange, S Tribble, RE Tribedy, P Trzeciak, BA Tsai, OD Turnau, J Ullrich, T Underwood, DG Van Buren, G van Nieuwenhuizen, G Vandenbroucke, M Vanfossen, JA Varma, R Vasconcelos, GMS Vasiliev, AN Vertesi, R Videbaek, F Viyogi, YP Vokal, S Vossen, A Wada, M Wang, F Wang, G Wang, H Wang, JS Wang, XL Wang, Y Wang, Y Webb, G Webb, JC Westfall, GD Wieman, H Wissink, SW Witt, R Wu, YF Xiao, Z Xie, W Xin, K Xu, H Xu, J Xu, N Xu, H Xu, Y Xu, Z Yan, W Yang, C Yang, Y Yang, Y Ye, Z Yepes, P Yi, L Yip, K Yoo, IK Yu, N Zbroszczyk, H Zha, W Zhang, JB Zhang, JL Zhang, S Zhang, XP Zhang, Y Zhang, ZP Zhao, F Zhao, J Zhong, C Zhu, X Zhu, YH Zoulkarneeva, Y Zyzak, M AF Adamczyk, L. Adkins, J. K. Agakishiev, G. Aggarwal, M. M. Ahammed, Z. Alekseev, I. Alford, J. Anson, C. D. Aparin, A. Arkhipkin, D. Aschenauer, E. C. Averichev, G. S. Banerjee, A. Beavis, D. R. Bellwied, R. Bhasin, A. Bhati, A. K. Bhattarai, P. Bichsel, H. Bielcik, J. Bielcikova, J. Bland, L. C. Bordyuzhin, I. G. Borowski, W. Bouchet, J. Brandin, A. V. Brovko, S. G. Bultmann, S. Bunzarov, I. Burton, T. P. Butterworth, J. Caines, H. Sanchez, M. Calderon de la Barca Campbell, J. M. Cebra, D. Cendejas, R. Cervantes, M. C. Chaloupka, P. Chang, Z. Chattopadhyay, S. Chen, H. F. Chen, J. H. Chen, L. Cheng, J. Cherney, M. Chikanian, A. Christie, W. Chwastowski, J. Codrington, M. J. M. Contin, G. Cramer, J. G. Crawford, H. J. Cui, X. Das, S. Leyva, A. Davila De Silva, L. C. Debbe, R. R. Dedovich, T. G. Deng, J. Derevschikov, A. A. Derradi de Souza, R. di Ruzza, B. Didenko, L. Dilks, C. Ding, F. Djawotho, P. Dong, X. Drachenberg, J. L. Draper, J. E. Du, C. M. Dunkelberger, L. E. Dunlop, J. C. Efimov, L. G. Engelage, J. Engle, K. S. Eppley, G. Eun, L. Evdokimov, O. Eyser, O. Fatemi, R. Fazio, S. Fedorisin, J. Filip, P. Fisyak, Y. Flores, C. E. Gagliardi, C. A. Gangadharan, D. R. Garand, D. Geurts, F. Gibson, A. Girard, M. Gliske, S. Greiner, L. Grosnick, D. Gunarathne, D. S. Guo, Y. Gupta, A. Gupta, S. Guryn, W. Haag, B. Hamed, A. Han, L-X. Haque, R. Harris, J. W. Heppelmann, S. Hirsch, A. Hoffmann, G. W. Hofman, D. J. Horvat, S. Huang, B. Huang, H. Z. Huang, X. Huck, P. Humanic, T. J. Igo, G. Jacobs, W. W. Jang, H. Judd, E. G. Kabana, S. Kalinkin, D. Kang, K. Kauder, K. Ke, H. W. Keane, D. Kechechyan, A. Kesich, A. Khan, Z. H. Kikola, D. P. Kisel, I. Kisiel, A. Koetke, D. D. Kollegger, T. Konzer, J. Koralt, I. Kosarzewski, L. K. Kotchenda, L. Kraishan, A. F. Kravtsov, P. Krueger, K. Kulakov, I. Kumar, L. Kycia, R. A. Lamont, M. A. C. Landgraf, J. M. Landry, K. D. Lauret, J. Lebedev, A. Lednicky, R. Lee, J. H. Li, C. Li, W. Li, X. Li, X. Li, Y. Li, Z. M. Lisa, M. A. Liu, F. Ljubicic, T. Llope, W. J. Lomnitz, M. Longacre, R. S. Luo, X. Ma, G. L. Ma, Y. G. Mahapatra, D. P. Majka, R. Margetis, S. Markert, C. Masui, H. Matis, H. S. McDonald, D. McShane, T. S. Minaev, N. G. Mioduszewski, S. Mohanty, B. Mondal, M. M. Morozov, D. A. Mustafa, M. K. Nandi, B. K. Nasim, Md. Nayak, T. K. Nelson, J. M. Nigmatkulov, G. Nogach, L. V. Noh, S. Y. Novak, J. Nurushev, S. B. Odyniec, G. Ogawa, A. Oh, K. Ohlson, A. Okorokov, V. Oldag, E. W. Olvitt, D. L., Jr. Page, B. S. Pan, Y. X. Pandit, Y. Panebratsev, Y. Pawlak, T. Pawlik, B. Pei, H. Perkins, C. Pile, P. Planinic, M. Pluta, J. Poljak, N. Poniatowska, K. Porter, J. Poskanzer, A. M. Pruthi, N. K. Przybycien, M. Putschke, J. Qiu, H. Quintero, A. Ramachandran, S. Raniwala, R. Raniwala, S. Ray, R. L. Riley, C. K. Ritter, H. G. Roberts, J. B. Rogachevskiy, O. V. Romero, J. L. Ross, J. F. Roy, A. Ruan, L. Rusnak, J. Rusnakova, O. Sahoo, N. R. Sahu, P. K. Sakrejda, I. Salur, S. Sandacz, A. Sandweiss, J. Sangaline, E. Sarkar, A. Schambach, J. Scharenberg, R. P. Schmah, A. M. Schmidke, W. B. Schmitz, N. Seger, J. Seyboth, P. Shah, N. Shahaliev, E. Shanmuganathan, P. V. Shao, M. Sharma, B. Shen, W. Q. Shi, S. S. Shou, Q. Y. Sichtermann, E. P. Simko, M. Skoby, M. J. Smirnov, D. Smirnov, N. Solanki, D. Sorensen, P. Spinka, H. M. Srivastava, B. Stanislaus, T. D. S. Stevens, J. R. Stock, R. Strikhanov, M. Stringfellow, B. Sumbera, M. Sun, X. Sun, X. M. Sun, Y. Sun, Z. Surrow, B. Svirida, D. N. Symons, T. J. M. Szelezniak, M. A. Takahashi, J. Tang, A. H. Tang, Z. Tarnowsky, T. Thomas, J. H. Timmins, A. R. Tlusty, D. Tokarev, M. Trentalange, S. Tribble, R. E. Tribedy, P. Trzeciak, B. A. Tsai, O. D. Turnau, J. Ullrich, T. Underwood, D. G. Van Buren, G. van Nieuwenhuizen, G. Vandenbroucke, M. Vanfossen, J. A., Jr. Varma, R. Vasconcelos, G. M. S. Vasiliev, A. N. Vertesi, R. Videbaek, F. Viyogi, Y. P. Vokal, S. Vossen, A. Wada, M. Wang, F. Wang, G. Wang, H. Wang, J. S. Wang, X. L. Wang, Y. Wang, Y. Webb, G. Webb, J. C. Westfall, G. D. Wieman, H. Wissink, S. W. Witt, R. Wu, Y. F. Xiao, Z. Xie, W. Xin, K. Xu, H. Xu, J. Xu, N. Xu, H. Xu, Y. Xu, Z. Yan, W. Yang, C. Yang, Y. Yang, Y. Ye, Z. Yepes, P. Yi, L. Yip, K. Yoo, I-K. Yu, N. Zbroszczyk, H. Zha, W. Zhang, J. B. Zhang, J. L. Zhang, S. Zhang, X. P. Zhang, Y. Zhang, Z. P. Zhao, F. Zhao, J. Zhong, C. Zhu, X. Zhu, Y. H. Zoulkarneeva, Y. Zyzak, M. CA STAR Collaboration TI Charged-to-neutral correlation at forward rapidity in Au plus Au collisions at root s(NN)=200 GeV SO PHYSICAL REVIEW C LA English DT Article ID DISORIENTED CHIRAL CONDENSATE; QUARK-GLUON PLASMA; TIME PROJECTION CHAMBER; HEAVY-ION COLLISIONS; STAR EXPERIMENT; FLUCTUATIONS; SEARCH; COLLABORATION; PERSPECTIVE; DETECTOR AB Event-by-event fluctuations of the multiplicities of inclusive charged particles and photons at forward rapidity in Au + Au collisions at root s(NN) = 200 GeV have been studied. The dominant contribution to such fluctuations is expected to come from correlated production of charged and neutral pions. We search for evidence of dynamical fluctuations of different physical origins. Observables constructed out of moments of multiplicities are used as measures of fluctuations. Mixed events and model calculations are used as base lines. Results are compared to the dynamical net-charge fluctuations measured in the same acceptance. A nonzero statistically significant signal of dynamical fluctuations is observed in excess to the model prediction when charged particles and photons are measured in the same acceptance. We find that, unlike dynamical net-charge fluctuation, charge-neutral fluctuation is not dominated by correlation owing to particle decay. Results are compared to the expectations based on the generic production mechanism of pions owing to isospin symmetry, for which no significant (<1%) deviation is observed. 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Calderon de la Barca; Cebra, D.; Ding, F.; Draper, J. E.; Flores, C. E.; Haag, B.; Kesich, A.; Romero, J. L.; Sangaline, E.] Univ Calif Davis, Davis, CA 95616 USA. [Dunkelberger, L. E.; Huang, H. Z.; Igo, G.; Landry, K. D.; Nasim, Md.; Pan, Y. X.; Shah, N.; Trentalange, S.; Tsai, O. D.; Wang, G.; Zhao, F.] Univ Calif Los Angeles, Los Angeles, CA 90095 USA. [Derradi de Souza, R.; Takahashi, J.; Vasconcelos, G. M. S.] Univ Estadual Campinas, Sao Paulo, Brazil. [Chen, L.; Huck, P.; Li, Z. M.; Liu, F.; Luo, X.; Pei, H.; Wu, Y. F.; Xu, J.; Yang, Y.; Yu, N.; Zhang, J. B.; Zhao, J.] Cent China Normal Univ HZNU, Wuhan 430079, Peoples R China. [Evdokimov, O.; Hofman, D. J.; Kauder, K.; Khan, Z. H.; Pandit, Y.; Wang, Y.; Ye, Z.] Univ Illinois, Chicago, IL 60607 USA. [Kycia, R. A.] Cracow Univ Technol, PL-30084 Krakow, Poland. [Cherney, M.; De Silva, L. C.; McShane, T. S.; Ross, J. F.; Seger, J.] Creighton Univ, Omaha, NE 68178 USA. 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[Cendejas, R.; Dilks, C.; Heppelmann, S.] Penn State Univ, University Pk, PA 16802 USA. [Derevschikov, A. A.; Minaev, N. G.; Morozov, D. A.; Nogach, L. V.; Nurushev, S. B.; Vasiliev, A. N.] Inst High Energy Phys, Protvino, Russia. [Derevschikov, A. A.; Garand, D.; Hirsch, A.; Konzer, J.; Li, X.; Scharenberg, R. P.; Srivastava, B.; Stringfellow, B.; Wang, F.; Xie, W.; Yi, L.] Purdue Univ, W Lafayette, IN 47907 USA. [Raniwala, R.; Raniwala, S.; Solanki, D.] Univ Rajasthan, Jaipur 302004, Rajasthan, India. [Butterworth, J.; Eppley, G.; Geurts, F.; Llope, W. J.; Roberts, J. B.; Xin, K.; Yepes, P.] Rice Univ, Houston, TX 77251 USA. [Chen, H. F.; Cui, X.; Guo, Y.; Li, C.; Shao, M.; Sun, Y.; Tang, Z.; Wang, X. L.; Xu, Y.; Yang, C.; Zha, W.; Zhang, Y.; Zhang, Z. P.] Univ Sci & Technol China, Anhua 230026, Peoples R China. [Deng, J.; Xu, H.; Zhang, J. L.] Shandong Univ, Jinan 250100, Shandong, Peoples R China. [Chen, J. H.; Han, L-X.; Li, W.; Ma, G. L.; Ma, Y. G.; Shen, W. Q.; Shou, Q. Y.; Zhang, S.; Zhong, C.; Zhu, Y. H.] Shanghai Inst Appl Phys, Shanghai 201800, Peoples R China. [Borowski, W.; Kabana, S.] SUBATECH, Nantes, France. [Gunarathne, D. S.; Kraishan, A. F.; Li, X.; Olvitt, D. L., Jr.; Surrow, B.; Vandenbroucke, M.] Temple Univ, Philadelphia, PA 19122 USA. [Cervantes, M. C.; Chang, Z.; Djawotho, P.; Gagliardi, C. A.; Hamed, A.; Mioduszewski, S.; Mondal, M. M.; Sahoo, N. R.; Tribble, R. E.] Texas A&M Univ, College Stn, TX 77843 USA. [Bhattarai, P.; Codrington, M. J. M.; Leyva, A. Davila; Hoffmann, G. W.; Markert, C.; Oldag, E. W.; Ray, R. L.; Schambach, J.; Wada, M.] Univ Texas Austin, Austin, TX 78712 USA. [Bellwied, R.; McDonald, D.; Timmins, A. R.] Univ Houston, Houston, TX 77204 USA. [Cheng, J.; Huang, X.; Kang, K.; Li, Y.; Wang, Y.; Xiao, Z.; Yan, W.; Zhang, X. P.; Zhu, X.] Tsinghua Univ, Beijing 100084, Peoples R China. [Engle, K. S.; Witt, R.] US Naval Acad, Annapolis, MD 21402 USA. [Drachenberg, J. L.; Gibson, A.; Grosnick, D.; Koetke, D. D.; Stanislaus, T. D. S.] Valparaiso Univ, Valparaiso, IN 46383 USA. [Ahammed, Z.; Banerjee, A.; Chattopadhyay, S.; Nayak, T. K.; Roy, A.; Tribedy, P.; Viyogi, Y. P.] Bhabha Atom Res Ctr, Ctr Variable Energy Cyclotron, Kolkata 700064, W Bengal, India. [Girard, M.; Kikola, D. P.; Kisiel, A.; Kosarzewski, L. K.; Pawlak, T.; Pluta, J.; Poniatowska, K.; Sandacz, A.; Zbroszczyk, H.] Warsaw Univ Technol, Warsaw, Poland. [Bichsel, H.; Cramer, J. G.] Univ Washington, Seattle, WA 98195 USA. [Putschke, J.] Wayne State Univ, Detroit, MI 48201 USA. [Caines, H.; Chikanian, A.; Harris, J. W.; Horvat, S.; Majka, R.; Ohlson, A.; Riley, C. K.; Sandweiss, J.; Smirnov, N.] Yale Univ, New Haven, CT 06520 USA. [Planinic, M.; Poljak, N.] Univ Zagreb, HR-10002 Zagreb, Croatia. RP Greiner, L (reprint author), AGH Univ Sci & Technol, PL-30059 Krakow, Poland. RI Chaloupka, Petr/E-5965-2012; Takahashi, Jun/B-2946-2012; Huang, Bingchu/H-6343-2015; Xin, Kefeng/O-9195-2016; Yi, Li/Q-1705-2016; Alekseev, Igor/J-8070-2014; Svirida, Dmitry/R-4909-2016; Kumar, Lokesh/A-6154-2010; Rusnak, Jan/G-8462-2014; Sumbera, Michal/O-7497-2014; Fazio, Salvatore /G-5156-2010; Kycia, Radoslaw/J-4397-2015; Bielcikova, Jana/G-9342-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Ma, Yu-Gang/M-8122-2013; Gunarathne, Devika/C-4903-2017; Derradi de Souza, Rafael/M-4791-2013 OI Takahashi, Jun/0000-0002-4091-1779; Huang, Bingchu/0000-0002-3253-3210; Xin, Kefeng/0000-0003-4853-9219; Yi, Li/0000-0002-7512-2657; Alekseev, Igor/0000-0003-3358-9635; Kumar, Lokesh/0000-0002-2746-9840; Sumbera, Michal/0000-0002-0639-7323; Kycia, Radoslaw/0000-0002-6390-4627; Ma, Yu-Gang/0000-0002-0233-9900; Gunarathne, Devika/0000-0002-7155-7418; Derradi de Souza, Rafael/0000-0002-2084-7001 FU Office of NP within the U.S. DOE Office of Science; Office of HEP within the U.S. DOE Office of Science; U.S. NSF; CNRS/IN2P3; FAPESP CNPq of Brazil; Ministry of Education and Science of the Russian Federation; NNSFC; CAS; MoST; MoE of China; Korean Research Foundation; GA and MSMT of the Czech Republic; FIAS of Germany; DAE; DST; CSIR of India; National Science Centre of Poland; National Research Foundation [NRF-2012004024]; Ministry of Science, Education and Sports of the Republic of Croatia; RosAtom of Russia FX We thank the RHIC Operations Group and RCF at BNL, the NERSC Center at LBNL, the KISTI Center in Korea, and the Open Science Grid consortium for providing resources and support. This work was supported in part by the Offices of NP and HEP within the U.S. DOE Office of Science, the U.S. NSF, CNRS/IN2P3; FAPESP CNPq of Brazil; the Ministry of Education and Science of the Russian Federation, NNSFC, CAS, MoST, and MoE of China; the Korean Research Foundation; GA and MSMT of the Czech Republic; FIAS of Germany; DAE, DST, and CSIR of India; the National Science Centre of Poland; National Research Foundation (NRF-2012004024); the Ministry of Science, Education and Sports of the Republic of Croatia; and RosAtom of Russia. NR 64 TC 1 Z9 1 U1 3 U2 37 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAR 20 PY 2015 VL 91 IS 3 AR 034905 DI 10.1103/PhysRevC.91.034905 PG 13 WC Physics, Nuclear SC Physics GA CE8GA UT WOS:000352078500002 ER PT J AU van der Laan, JD Scrymgeour, DA Kemme, SA Dereniak, EL AF van der Laan, J. D. Scrymgeour, D. A. Kemme, S. A. Dereniak, E. L. TI Detection range enhancement using circularly polarized light in scattering environments for infrared wavelengths SO APPLIED OPTICS LA English DT Article ID BACKSCATTERING TARGET DETECTION; IMAGING POLARIMETRY; TURBID MEDIUM; MEDIA; WAVES; FOG; DISCRIMINATION; DUST AB We find for infrared wavelengths that there are broad ranges of particle sizes and refractive indices that represent fog and rain, where circular polarization can persist to longer ranges than linear polarization. Using polarization tracking Monte Carlo simulations for varying particle size, wavelength, and refractive index, we show that, for specific scene parameters, circular polarization outperforms linear polarization in maintaining the illuminating polarization state for large optical depths. This enhancement with circular polarization can be exploited to improve range and target detection in obscurant environments that are important in many critical sensing applications. Initially, researchers employed polarization-discriminating schemes, often using linearly polarized active illumination, to further distinguish target signals from the background noise. More recently, researchers have investigated circular polarization as a means to separate signal from noise even more. Specifically, we quantify both linearly and circularly polarized active illumination and show here that circular polarization persists better than linear for radiation fog in the short-wave infrared, for advection fog in the short-wave and long-wave infrared, and large particle sizes of Sahara dust around the 4 mu m wavelength. Conversely, we quantify where linear polarization persists better than circular polarization for some limited particle sizes of radiation fog in the long-wave infrared, small particle sizes of Sahara dust for wavelengths of 9-10.5 mu m, and large particle sizes of Sahara dust through the 8-11 mu m wavelength range in the long-wave infrared. (c) 2015 Optical Society of America C1 [van der Laan, J. D.; Dereniak, E. L.] Univ Arizona, Ctr Opt Sci, Tucson, AZ 85721 USA. [van der Laan, J. D.; Scrymgeour, D. A.; Kemme, S. A.] Sandia Natl Labs, Albuquerque, NM 87123 USA. RP van der Laan, JD (reprint author), Univ Arizona, Ctr Opt Sci, 1630 E Univ Blvd, Tucson, AZ 85721 USA. EM jdvander@optics.arizona.edu RI Scrymgeour, David/C-1981-2008 FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 30 TC 7 Z9 7 U1 1 U2 18 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1559-128X EI 2155-3165 J9 APPL OPTICS JI Appl. Optics PD MAR 20 PY 2015 VL 54 IS 9 BP 2266 EP 2274 DI 10.1364/AO.54.002266 PG 9 WC Optics SC Optics GA CE2IC UT WOS:000351638300014 PM 25968509 ER PT J AU Bernacki, BE Douglas, M Erchinger, JL Fuller, ES Keillor, ME Morley, SM Mullen, CA Orrell, JL Panisko, ME Warren, GA Wright, ME AF Bernacki, Bruce E. Douglas, Matthew Erchinger, Jennifer L. Fuller, Erin S. Keillor, Martin E. Morley, Shannon M. Mullen, Crystal A. Orrell, John L. Panisko, Mark E. Warren, Glen A. Wright, Michael E. TI Optical design considerations for efficient light collection from liquid scintillation counters SO APPLIED OPTICS LA English DT Article AB Liquid scintillation counters measure charged particle-emitting radioactive isotopes and are used for environmental studies, nuclear chemistry, and life science. Alpha and beta emissions arising from the material under study interact with the scintillation cocktail to produce light. The prototypical liquid scintillation counter employs low-level photon-counting detectors to measure the arrival of the scintillation. For reliable operation, the counting instrument must convey the scintillation light to the detectors efficiently and predictably. Current best practices employ the use of two or more detectors for coincidence processing to discriminate true scintillation events from background events due to instrumental effects such as photomultiplier tube dark rates, tube flashing, or other light emission not generated in the scintillation cocktail vial. In low-background liquid scintillation counters, additional attention is paid to shielding the scintillation cocktail from naturally occurring radioactive material present in the laboratory and within the instrument's construction materials. Low-background design is generally at odds with optimal light collection. This study presents the evolution of a light collection design for liquid scintillation counting (LSC) in a low-background shield. The basic approach to achieve both good light collection and a low-background measurement is described. The baseline signals arising from the scintillation vial are modeled and methods to efficiently collect scintillation light are presented as part of the development of a customized low-background, high-sensitivity LSC system. C1 [Bernacki, Bruce E.; Douglas, Matthew; Erchinger, Jennifer L.; Fuller, Erin S.; Keillor, Martin E.; Morley, Shannon M.; Mullen, Crystal A.; Orrell, John L.; Panisko, Mark E.; Warren, Glen A.; Wright, Michael E.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Erchinger, Jennifer L.] Texas A&M Univ, College Stn, TX 77843 USA. RP Bernacki, BE (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM bruce.bernacki@pnnl.gov RI Orrell, John/E-9313-2015; OI Orrell, John/0000-0001-7968-4051; Douglas, Matthew/0000-0001-9708-1780 NR 13 TC 0 Z9 0 U1 0 U2 4 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1559-128X EI 2155-3165 J9 APPL OPTICS JI Appl. Optics PD MAR 20 PY 2015 VL 54 IS 9 BP 2413 EP 2423 DI 10.1364/AO.54.002413 PG 11 WC Optics SC Optics GA CE2IC UT WOS:000351638300035 PM 25968530 ER PT J AU Boley, CD Khairallah, SA Rubenchik, AM AF Boley, C. D. Khairallah, S. A. Rubenchik, A. M. TI Calculation of laser absorption by metal powders in additive manufacturing SO APPLIED OPTICS LA English DT Article ID SIMULATION; MODEL AB We have calculated the absorption of laser light by a powder of metal spheres, typical of the powder employed in laser powder-bed fusion additive manufacturing. Using ray-trace simulations, we show that the absorption is significantly larger than its value for normal incidence on a flat surface, due to multiple scattering. We investigate the dependence of absorption on powder content (material, size distribution, and geometry) and on beam size. (c) 2015 Optical Society of America C1 [Boley, C. D.; Khairallah, S. A.; Rubenchik, A. M.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Boley, CD (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM boley1@llnl.gov FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Laboratory Directed Research and Development Program at Lawrence Livermore National Laboratory [13-SI-002] FX We would like to thank W. E. King and W. A. Molander for helpful discussions. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. This work was funded by the Laboratory Directed Research and Development Program at Lawrence Livermore National Laboratory under project tracking code 13-SI-002. NR 14 TC 14 Z9 15 U1 8 U2 54 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1559-128X EI 2155-3165 J9 APPL OPTICS JI Appl. Optics PD MAR 20 PY 2015 VL 54 IS 9 BP 2477 EP 2482 DI 10.1364/AO.54.002477 PG 6 WC Optics SC Optics GA CE2IC UT WOS:000351638300042 PM 25968537 ER PT J AU Craig, N Knapen, S Longhi, P AF Craig, Nathaniel Knapen, Simon Longhi, Pietro TI The Orbifold Higgs SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Discrete and Finite Symmetries; Global Symmetries; Large Extra Dimensions ID GRAND UNIFICATION; EXTRA DIMENSIONS; FIELD-THEORIES; BREAKING; BOSON; MASS; LHC; GUT AB We introduce and systematically study an expansive class of "orbifold Higgs" theories in which the weak scale is protected by accidental symmetries arising from the orbifold reduction of continuous symmetries. The protection mechanism eliminates quadratic sensitivity of the Higgs mass to higher scales at one loop (or more) and does not involve any new states charged under the Standard Model. The structures of the Higgs and top sectors are universal and determined exclusively by group theoretical considerations. The twin Higgs model fits within our framework as the simplest example of an orbifold Higgs. Our models admit UV completions as geometric orbifolds in higher dimensions, and fit naturally within frameworks of low scale gauge coupling unification. C1 [Craig, Nathaniel] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA. [Knapen, Simon] Univ Calif Berkeley, Berkeley Ctr Theoret Phys, Berkeley, CA 94720 USA. [Knapen, Simon] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Theoret Phys Grp, Berkeley, CA 94720 USA. [Longhi, Pietro] Rutgers State Univ, New High Energy Theory Ctr, Piscataway, NJ 08854 USA. RP Craig, N (reprint author), Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA. EM ncraig@physics.ucsb.edu; smknapen@lbl.gov; longhi@physics.rutgers.edu FU DOE [SC0010008, ARRA-SC0003883, DE-SC0007897]; Aspen Center for Physics; NSF [1066293]; U.S. Department of Energy [DE-AC02-05CH11231] FX We thank Aria Basirnia, Zackaria Chacko, Aleksey Cherman, Tony Gherghetta, Roni Harnik, Kiel Howe, Andrey Katz, Alberto Mariotti, Yasunori Nomura, Duccio Pappadopulo, Michele Papucci, Gilad Perez, Stuart Raby, Michael Ratz, Michele Redi, Martin Schmaltz, Raman Sundrum, and Jure Zupan for helpful discussions. We especially thank Matt Strassler both for particularly useful conversations and for asking the question, "how do you generalize the Twin Higgs?" This work was supported in part by DOE grants SC0010008, ARRA-SC0003883, and DE-SC0007897. N.C. acknowledges support from the Aspen Center for Physics and NSF grant 1066293 where this work was partially completed. This manuscript has been authored by an author (SK) at Lawrence Berkeley National Laboratory under Contract No. DE-AC02-05CH11231 with the U.S. Department of Energy. The U.S. Government retains, and the publisher, by accepting the article for publication, acknowledges, that the U.S. Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for U.S. Government purposes. NR 49 TC 24 Z9 24 U1 0 U2 2 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAR 20 PY 2015 IS 3 AR 106 DI 10.1007/JHEP03(2015)106 PG 40 WC Physics, Particles & Fields SC Physics GA CD8US UT WOS:000351372500002 ER PT J AU Xiong, JB He, ZL Shi, SJ Kent, A Deng, Y Wu, LY Van Nostrand, JD Zhou, JZ AF Xiong, Jinbo He, Zhili Shi, Shengjing Kent, Angela Deng, Ye Wu, Liyou Van Nostrand, Joy D. Zhou, Jizhong TI Elevated CO2 shifts the functional structure and metabolic potentials of soil microbial communities in a C-4 agroecosystem SO SCIENTIFIC REPORTS LA English DT Article ID ATMOSPHERIC CO2; CARBON-DIOXIDE; NITROGEN LIMITATION; FOREST PRODUCTIVITY; ENRICHMENT FACE; GRASSLAND SOIL; RESPONSES; MAIZE; PHOTOSYNTHESIS; METAANALYSIS AB Atmospheric CO2 concentration is continuously increasing, and previous studies have shown that elevated CO2 (eCO(2)) significantly impacts C-3 plants and their soil microbial communities. However, little is known about effects of eCO(2) on the compositional and functional structure, and metabolic potential of soil microbial communities under C-4 plants. Here we showed that a C-4 maize agroecosystem exposed to eCO(2) for eight years shifted the functional and phylogenetic structure of soil microbial communities at both soil depths (0-5 cm and 5-15 cm) using EcoPlate and functional gene array (GeoChip 3.0) analyses. The abundances of key genes involved in carbon (C), nitrogen (N) and phosphorus (P) cycling were significantly stimulated under eCO(2) at both soil depths, although some differences in carbon utilization patterns were observed between the two soil depths. Consistently, CO2 was found to be the dominant factor explaining 11.9% of the structural variation of functional genes, while depth and the interaction of depth and CO2 explained 5.2% and 3.8%, respectively. This study implies that eCO(2) has profound effects on the functional structure and metabolic potential/ activity of soil microbial communities associated with C-4 plants, possibly leading to changes in ecosystem functioning and feedbacks to global change in C-4 agroecosystems. C1 [Xiong, Jinbo] Ningbo Univ, Fac Marine Sci, Ningbo 315211, Zhejiang, Peoples R China. [Xiong, Jinbo; He, Zhili; Shi, Shengjing; Deng, Ye; Wu, Liyou; Van Nostrand, Joy D.; Zhou, Jizhong] Univ Oklahoma, Inst Environm Genom, Norman, OK 73019 USA. [Xiong, Jinbo; He, Zhili; Shi, Shengjing; Deng, Ye; Wu, Liyou; Van Nostrand, Joy D.; Zhou, Jizhong] Univ Oklahoma, Dept Microbiol & Plant Biol, Norman, OK 73019 USA. [Shi, Shengjing] Univ Calif Berkeley, Dept Environm Sci Policy & Management, Berkeley, CA 94720 USA. [Kent, Angela] Univ Illinois, Dept Nat Resources & Environm Sci, Urbana, IL 61820 USA. [Deng, Ye] Chinese Acad Sci, Res Ctr Ecoenvironm Sci, Key Lab Environm Biotechnol, Beijing 100085, Peoples R China. [Zhou, Jizhong] Tsinghua Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100084, Peoples R China. [Zhou, Jizhong] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Earth Sci Div, Berkeley, CA 94720 USA. RP He, ZL (reprint author), Univ Oklahoma, Inst Environm Genom, Norman, OK 73019 USA. EM zhili.he@ou.edu; jzhou@ou.edu RI Van Nostrand, Joy/F-1740-2016; OI Van Nostrand, Joy/0000-0001-9548-6450; ?, ?/0000-0002-7584-0632 FU US Department of Agriculture through the NSF-USDA Microbial Observatories Program [2007-35319-18305]; Oklahoma Applied Research Support (OARS), Oklahoma Center for the Advancement of Science and Technology (OCAST) [AR062-034, AR11-035]; KC Wong Magna Fund of Ningbo University FX Assistance with sample collection was provided by Ariane L. Peralta, Yu-rui Chang, Sara F. Paver, Diana N. Flanagan, and Anthony C. Yannarell. This work is supported by the US Department of Agriculture (Project 2007-35319-18305) through the NSF-USDA Microbial Observatories Program, and by Oklahoma Applied Research Support (OARS), Oklahoma Center for the Advancement of Science and Technology (OCAST) through AR062-034 and AR11-035, and the KC Wong Magna Fund of Ningbo University. NR 59 TC 5 Z9 5 U1 2 U2 44 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAR 20 PY 2015 VL 5 AR 9316 DI 10.1038/srep09316 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CD7RQ UT WOS:000351289300001 PM 25791904 ER PT J AU Kung, HH Baumbach, RE Bauer, ED Thorsmolle, VK Zhang, WL Haule, K Mydosh, JA Blumberg, G AF Kung, H. -H. Baumbach, R. E. Bauer, E. D. Thorsmolle, V. K. Zhang, W. -L. Haule, K. Mydosh, J. A. Blumberg, G. TI Chirality density wave of the "hidden order" phase in URu2Si2 SO SCIENCE LA English DT Article ID SYMMETRY-BREAKING; RAMAN-SCATTERING; SUPERCONDUCTOR URU2SI2; MAGNETIC EXCITATIONS; FERMI-SURFACE; SYSTEMS; LATTICE; TRANSITION; ENTROPY AB A second-order phase transition in a physical system is associated with the emergence of an "order parameter" and a spontaneous symmetry breaking. The heavy fermion superconductor URu2Si2 has a "hidden order" (HO) phase below the temperature of 17.5 kelvin; the symmetry of the associated order parameter has remained ambiguous. Here we use polarization-resolved Raman spectroscopy to specify the symmetry of the low-energy excitations above and below the HO transition. We determine that the HO parameter breaks local vertical and diagonal reflection symmetries at the uranium sites, resulting in crystal field states with distinct chiral properties, which order to a commensurate chirality density wave ground state. C1 [Kung, H. -H.; Thorsmolle, V. K.; Zhang, W. -L.; Haule, K.; Blumberg, G.] Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08854 USA. [Baumbach, R. E.; Bauer, E. D.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Mydosh, J. A.] Leiden Univ, Kamerlingh Onnes Lab, NL-2300 RA Leiden, Netherlands. [Blumberg, G.] NICPB, EE-12618 Tallinn, Estonia. RP Blumberg, G (reprint author), Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08854 USA. EM skung@physics.rutgers.edu; haule@physics.rutgers.edu; girsh@physics.rutgers.edu RI Thorsmolle, Verner/M-1095-2015; Kung, Hsiang-Hsi/R-4949-2016; OI Thorsmolle, Verner/0000-0002-5890-4403; Kung, Hsiang-Hsi/0000-0002-2835-3196; Bauer, Eric/0000-0003-0017-1937 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-SC0005463]; National Science Foundation under Award NSF [DMR-1104884]; NSF [DMR-1405303]; Institute for Complex Adaptive Matter (NSF-IMI) [DMR-0844115] FX We thank J. Buhot, P. Chandra, P. Coleman, G. Kotliar, M.-A. Measson, D. K. Morr, L. Pascut, A. Sacuto, J. Thompson, and V. M. Yakovenko for discussions. G.B. and V.K.T. acknowledge support from the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Award DE-SC0005463. H.-H. K. acknowledges support from the National Science Foundation under Award NSF DMR-1104884. K.H. acknowledges support by NSF DMR-1405303. W.-L.Z. acknowledges support by the Institute for Complex Adaptive Matter (NSF-IMI grant DMR-0844115). Work at Los Alamos National Laboratory was performed under the auspices of the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. NR 31 TC 19 Z9 19 U1 12 U2 58 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD MAR 20 PY 2015 VL 347 IS 6228 BP 1339 EP 1342 DI 10.1126/science.1259729 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CD6SM UT WOS:000351219600035 PM 25678557 ER PT J AU Timilsina, R Tan, S Livengood, R Rack, PD AF Timilsina, R. Tan, S. Livengood, R. Rack, P. D. TI Monte Carlo simulations of nanoscale focused neon ion beam sputtering of copper: elucidating resolution limits and sub-surface damage (vol 25, 485704, 2014) SO NANOTECHNOLOGY LA English DT Correction C1 [Timilsina, R.; Rack, P. D.] Univ Tennessee, Knoxville, TN 37996 USA. [Tan, S.; Livengood, R.] Intel Corp, Santa Clara, CA 95054 USA. [Rack, P. D.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Timilsina, R (reprint author), Univ Tennessee, Knoxville, TN 37996 USA. EM rtimilsi@utk.edu NR 1 TC 0 Z9 0 U1 2 U2 5 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 EI 1361-6528 J9 NANOTECHNOLOGY JI Nanotechnology PD MAR 20 PY 2015 VL 26 IS 11 AR 119501 DI 10.1088/0957-4484/26/11/119501 PG 2 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA CC7SO UT WOS:000350568900020 ER PT J AU Hu, MS Wang, Y Rutqvist, J AF Hu, Mengsu Wang, Yuan Rutqvist, Jonny TI An effective approach for modeling fluid flow in heterogeneous media using numerical manifold method SO INTERNATIONAL JOURNAL FOR NUMERICAL METHODS IN FLUIDS LA English DT Article DE heterogeneous media; fluid flow; jump function; numerical manifold method; refraction law; Lagrange multiplier method ID FINITE COVER METHOD; STATE GROUNDWATER-FLOW; POROUS-MEDIA; ELEMENT METHOD; SOLIDS; DISCONTINUITIES; SIMULATION; PARTITION; FRACTURE; VELOCITY AB A major challenge of modeling fluid flow in heterogeneous media is to model the material interfaces, which may be arbitrarily oriented or intersected with Dirichlet, Neumann, or other boundaries, making it difficult to mesh and accurately satisfy the boundary constraints. In order to solve these problems, we derived a new continuous approach in the numerical manifold method (NMM). NMM is an ideal method to handle boundaries, considering its flexibility and efficiency with fixed mathematical mesh and its integration precision. With the two-cover-meshing system, we construct physical covers containing gradient jump terms defined as extended degrees of freedom to realize the refraction law across material interfaces. In the global equilibrium equations, the jump terms are naturally considered with the energy-work seepage model. In this approach, high accuracy is expected from the newly constructed jump function together with simplex integration. Moreover, high mesh efficiency is realized by fixed triangular mathematical mesh with algorithms fully considering interfaces intersecting with Dirichlet, Neumann, or other boundaries and simplex integration on elements in arbitrary shapes. The new approach was coded into our NMM fluid flow model. We calculated examples involving fluid flow through a domain including (1) a single interface, (2) an idealized fault represented by multiple material interfaces, (3) intersected interfaces, and (4) an octagonal inclusion. We compared the simulated results to analytical solutions or results with denser mesh to test precision and efficiency and thereby proved that the new approach is accurate, efficient, and flexible, especially when considering intense geometric change or intersections. Copyright (c) 2015 John Wiley & Sons, Ltd. C1 [Hu, Mengsu; Wang, Yuan] Hohai Univ, Coll Civil & Transportat Engn, Nanjing 210098, Jiangsu, Peoples R China. [Hu, Mengsu; Wang, Yuan; Rutqvist, Jonny] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Wang, Y (reprint author), Hohai Univ, Coll Civil & Transportat Engn, Nanjing 210098, Jiangsu, Peoples R China. EM wangyuanhhu@163.com RI Rutqvist, Jonny/F-4957-2015; Hu, Mengsu/O-6202-2016 OI Rutqvist, Jonny/0000-0002-7949-9785; Hu, Mengsu/0000-0002-8853-2022 FU National Natural Science Foundation [51179060]; Education Ministry Foundation of China [20110094130002]; Graduates Science Innovation Research Project of Jiangsu Province [CXZZ12_0230]; China Scholarship Council; Program for Changjiang Scholars and Innovative Research Team in University [IRT1125]; 111 Project [B13024]; US Department of Energy [DE-AC02-05CH11231] FX The research was supported by the National Natural Science Foundation (No. 51179060), the Education Ministry Foundation of China (No. 20110094130002), the Graduates Science Innovation Research Project of Jiangsu Province (No. CXZZ12_0230), the China Scholarship Council, and in part, supported by the Program for Changjiang Scholars and Innovative Research Team in University (No. IRT1125), the 111 Project (No. B13024), and the US Department of Energy under contract No. DE-AC02-05CH11231. NR 33 TC 0 Z9 0 U1 3 U2 19 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0271-2091 EI 1097-0363 J9 INT J NUMER METH FL JI Int. J. Numer. Methods Fluids PD MAR 20 PY 2015 VL 77 IS 8 BP 459 EP 476 DI 10.1002/fld.3986 PG 18 WC Computer Science, Interdisciplinary Applications; Mathematics, Interdisciplinary Applications; Mechanics; Physics, Fluids & Plasmas SC Computer Science; Mathematics; Mechanics; Physics GA CB8RB UT WOS:000349897300002 ER PT J AU Saha, P Jampani, PH Datta, MK Hong, D Okoli, CU Manivannan, A Kumta, PN AF Saha, Partha Jampani, Prashanth H. Datta, Moni K. Hong, Daeho Okoli, Chris U. Manivannan, Ayyakkannu Kumta, Prashant N. TI Electrochemical Performance of Chemically and Solid State-Derived Chevrel Phase Mo6T8 (T = S, Se) Positive Electrodes for Sodium-Ion Batteries SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID CLUSTER CHALCOGENIDES MO6X8; ELECTRICAL ENERGY-STORAGE; RECHARGEABLE NA BATTERIES; HIGH-CAPACITY; AQUEOUS-ELECTROLYTE; PHYSICAL-PROPERTIES; LITHIUM; INTERCALATION; NA0.44MNO2; MECHANISM AB Chevrel phases, or CPs (Mo6T8; T = S, Se), can accommodate cations (Li+, Mg2+ etc.) within the Mo6T8 open framework at room temperature due to their unusually high electronic conductivity and ionic mobility and are hence proposed as positive electrodes for secondary batteries. However, cation insertion into Mo6T8 generates strong repulsion between the cation cation or cation-Mo atoms, leading to partial charge trapping within the Mo6T8 structure. The present work examines CPs as positive electrodes for Sodium-ion batteries. In this regard, ternary CPs of CuxMo6S8 and CuxMo6Se8 phase were prepared by solution chemistry and high energy mechanical milling (HEMM) routes, respectively, followed by acid leaching of copper. X-ray diffraction and scanning electron micrographs revealed the formation of 1-1.5 mu m size cuboidal Cu1.8Mo6S8 particles, whereas, HEMM of CuSe, MoSe2 and Mo powder followed by heating leads to the formation of Cu2Mo6Se8 phase. Results from cyclic voltammetry and galvanostatic cycling of Na/Mo6S8 and Na/Mo6Se8 cells within 1.22.2 V versus sodium revealed that two-step sodiation/desodiation reaction occurs with a gradual capacity fade due to Na-ion trapping within two terminal compositions, NaxMo6T8 (T = S, Se; x similar to 1 and 3). Electrochemical impedance spectroscopy at similar to 0.1 V intervals during the sodiation/desodiation process illustrates that partial Na-ion trapping, resulted in an increase in charge transfer resistance, R-e, due to the formation of stable Na similar to 1Mo6S8 phase after the first charge cycle. However, charge trapping continues to occur during the first and second cycles in the case of Mo6Se8 phase. Nevertheless, the ease: of fabrication, stable capacity, and high Coulombic efficiency render Mo6T8 (T = 8, Se) as promising Na-ion positive electrodes for stationary electrical energy storage (EES) applications. C1 [Saha, Partha; Jampani, Prashanth H.; Datta, Moni K.; Hong, Daeho; Kumta, Prashant N.] Univ Pittsburgh, Swanson Sch Engn, Dept Bioengn, Pittsburgh, PA 15261 USA. [Manivannan, Ayyakkannu] US DOE, Natl Energy Technol, Morgantown, WV 26507 USA. [Kumta, Prashant N.] Univ Pittsburgh, Swanson Sch Engn, Mech Engn & Mat Sci, Pittsburgh, PA 15261 USA. [Okoli, Chris U.; Kumta, Prashant N.] Univ Pittsburgh, Swanson Sch Engn, Chem & Petr Engn, Pittsburgh, PA 15261 USA. [Kumta, Prashant N.] Univ Pittsburgh, Sch Dent Med, Pittsburgh, PA 15261 USA. [Manivannan, Ayyakkannu] Univ Pittsburgh, Ctr Complex Engn Multifunct Mat, Pittsburgh, PA 15261 USA. RP Kumta, PN (reprint author), Univ Pittsburgh, Dept Bioengn, 815C Benedum Hall,3700 OHara St, Pittsburgh, PA 15261 USA. EM pkumta@pitt.edu RI SAHA, PARTHA/D-5508-2011; Jampani Hanumantha, Prashanth/A-9840-2013 OI SAHA, PARTHA/0000-0002-0309-8387; Jampani Hanumantha, Prashanth/0000-0001-7159-1993 FU U.S. Department of Energy [DE-AC02-05CH11231, 6951369]; Ford Foundation; Edward R. Weidlein Chair Professorship funds; Center for Complex Engineered Multifunctional Materials (CCEMM) FX The authors gratefully acknowledge the financial support provided by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231, Subcontract No. 6951369 under the Batteries for Advanced Transportation Technologies (BATT) program. The authors also acknowledge the National Science Foundation (NSF-CBET-0933141) and partial support of the Ford Foundation. P.N.K. also acknowledges the Edward R. Weidlein Chair Professorship funds and the Center for Complex Engineered Multifunctional Materials (CCEMM) for partial support of this research. NR 64 TC 7 Z9 7 U1 18 U2 81 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAR 19 PY 2015 VL 119 IS 11 BP 5771 EP 5782 DI 10.1021/jp509057w PG 12 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CE1FP UT WOS:000351557800003 ER PT J AU Romonosky, DE Laskin, A Laskin, J Nizkorodov, SA AF Romonosky, Dian E. Laskin, Alexander Laskin, Julia Nizkorodov, Sergey A. TI High-Resolution Mass Spectrometry and Molecular Characterization of Aqueous Photochemistry Products of Common Types of Secondary Organic Aerosols SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID BROWN CARBON; OPTICAL-PROPERTIES; HYDROGEN-PEROXIDE; SOA FORMATION; ORGANOSULFATES; PARTICLES; ISOPRENE; PHOTOOXIDATION; OZONOLYSIS; OXIDATION AB This work presents a systematic investigation of the molecular level composition and the extent of aqueous photochemical processing in different types of secondary organic aerosol (SOA) from biogenic and anthropogenic precursors including a-pinene, beta-pinene, beta-myrcene, D-limonene, alpha-humulene, 1,3,5-trimethylbenzene, and guaiacol, oxidized by ozone (to simulate a remote atmosphere) or by OH in the presence of NOx (to simulate an urban atmosphere). Chamber- and flow-tube-generated SOA samples were collected, extracted in a methanol/water solution, and photolyzed for 1 h under identical irradiation conditions. In these experiments, the irradiation was equivalent to about 3-8 h of exposure to the sun in its zenith. The molecular level composition of the dissolved SOA was probed before and after photolysis with direct-infusion electrospray ionization high-resolution mass spectrometry (ESI-HR-MS). The mass spectra of unphotolyzed SOA generated by ozone oxidation of monoterpenes showed qualitatively similar features and contained largely overlapping subsets of identified compounds. The mass spectra of OH/NOx-generated SOA had more unique visual appearance and indicated a lower extent of product overlap. Furthermore, the fraction of nitrogen-containing species (organonitrates and nitroaromatics) was highly sensitive to the SOA precursor. These observations suggest that attribution of high-resolution mass spectra in field SOA samples to specific SOA precursors should be more straightforward under OH/NOx oxidation conditions compared to the ozone-driven oxidation. Comparison of the SOA constituents before and after photolysis showed the tendency to reduce the average number of atoms in the SOA compounds without a significant effect on the overall O/C and H/C ratios. SOA prepared by OH/NOx photooxidation of 1,3,5-trimethylbenzene and guaiacol were more resilient to photolysis despite being the most light-absorbing. The composition of SOA prepared by ozonolysis of monoterpenes changed more significantly as a result of the photolysis. The results indicate that aqueous photolysis of dissolved SOA compounds in cloud/fog water can occur in various types of SOA, and on atmospherically relevant time scales. However, the extent of the photolysis-driven change in molecular composition depends on the specific type of SOA. C1 [Romonosky, Dian E.; Nizkorodov, Sergey A.] Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA. [Laskin, Alexander] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Laskin, Julia] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. RP Nizkorodov, SA (reprint author), Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA. EM nizkorod@uci.edu RI Laskin, Julia/H-9974-2012; Laskin, Alexander/I-2574-2012; Nizkorodov, Sergey/I-4120-2014 OI Laskin, Julia/0000-0002-4533-9644; Laskin, Alexander/0000-0002-7836-8417; Nizkorodov, Sergey/0000-0003-0891-0052 FU NSF [AGS-1227579]; Chemical Sciences Division, Office of Basic Energy Sciences of the U.S. DOE; Laboratory Directed Research and Development program of the W.R. Wiley Environmental Molecular Sciences Laboratory (EMSL)-a national scientific user facility located at PNNL; Office of Biological and Environmental Research of the U.S. PNNL for U.S. DOE [DE-AC06-76RL0 1830] FX We thank Dr. Hanna Lignell for help with actinometry measurements. The UCI group acknowledges support by the NSF Grant AGS-1227579. D.E.R. thanks NSF for the support via the graduate fellowship program. The PNNL group acknowledges support from the Chemical Sciences Division (J.L.), Office of Basic Energy Sciences of the U.S. DOE, and Laboratory Directed Research and Development program (A.L.) of the W.R. Wiley Environmental Molecular Sciences Laboratory (EMSL)-a national scientific user facility located at PNNL, and sponsored by the Office of Biological and Environmental Research of the U.S. PNNL is operated for U.S. DOE by Battelle Memorial Institute under Contract No. DE-AC06-76RL0 1830. NR 89 TC 10 Z9 10 U1 20 U2 119 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD MAR 19 PY 2015 VL 119 IS 11 SI SI BP 2594 EP 2606 DI 10.1021/jp509476r PG 13 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CE1FK UT WOS:000351557300045 PM 25412112 ER PT J AU Vanko, G Bordage, A Papai, M Haldrup, K Glatzel, P March, AM Doumy, G Britz, A Galler, A Assefa, T Cabaret, D Juhin, A van Driel, TB Kjaer, KS Dohn, A Moller, KB Lemke, HT Gallo, E Rovezzi, M Nemeth, Z Rozsalyi, E Rozgonyi, T Uhlig, J Sundstrom, V Nielsen, MM Young, L Southworth, SH Bressler, C Gawelda, W AF Vanko, Gyoergy Bordage, Amelie Papai, Matyas Haldrup, Kristoffer Glatzel, Pieter March, Anne Marie Doumy, Gilles Britz, Alexander Galler, Andreas Assefa, Tadesse Cabaret, Delphine Juhin, Amelie van Driel, Tim B. Kjaer, Kasper S. Dohn, Asmus Moller, Klaus B. Lemke, Henrik T. Gallo, Erik Rovezzi, Mauro Nemeth, Zoltan Rozsalyi, Emese Rozgonyi, Tams Uhlig, Jens Sundstrom, Villy Nielsen, Martin M. Young, Linda Southworth, Stephen H. Bressler, Christian Gawelda, Wojciech TI Detailed Characterization of a Nanosecond-Lived Excited State: X-ray and Theoretical Investigation of the Quintet State in Photoexcited [Fe(terpy)(2)](2+) SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID INDUCED SPIN-CROSSOVER; NEAR-EDGE STRUCTURE; ABSORPTION SPECTROSCOPY; BOND ORDER; PRE-EDGE; 1ST-PRINCIPLES CALCULATIONS; EMISSION SPECTROSCOPY; ELECTRONIC-STRUCTURE; PERTURBATION-THEORY; IRON(II) COMPLEX AB Theoretical predictions show that depending on the populations of the Fe 3d(xy), 3d(xz), and 3d(yz) orbitals two possible quintet states can exist for the high-spin state of the photoswitchable model system [Fe(terpy)(2)](2+). The differences in the structure and molecular properties of these B-5(2) and E-5 quintets are very small and pose a substantial challenge for experiments to resolve them. Yet for a better understanding of the physics of this system, which can lead to the design of novel molecules with enhanced photoswitching performance, it is vital to determine which high-spin state is reached in the transitions that follow the light excitation. The quintet state can be prepared with a short laser pulse and can be studied with cutting-edge time-resolved X-ray techniques. Here we report on the application of an extended set of X-ray spectroscopy and scattering techniques applied to investigate the quintet state of [Fe(terpy)(2)](2+) 80 ps after light excitation. High-quality X-ray absorption, nonresonant emission, and resonant emission spectra as well as X-ray diffuse scattering data clearly reflect the formation of the high-spin state of the [Fe(terpy)(2)](2+) molecule; moreover, extended X-ray absorption fine structure spectroscopy resolves the Fe-ligand bond-length variations with unprecedented bond-length accuracy in time-resolved experiments. With ab initio calculations we determine why, in contrast to most related systems, one configurational mode is insufficient for the description of the low-spin (LS)-high-spin (HS) transition. We identify the electronic structure origin of the differences between the two possible quintet modes, and finally, we unambiguously identify the formed quintet state as 5E, in agreement with our theoretical expectations. C1 [Vanko, Gyoergy; Bordage, Amelie; Papai, Matyas; Nemeth, Zoltan; Rozsalyi, Emese] Hungarian Acad Sci, Wigner Res Ctr Phys, POB 49, H-1525 Budapest, Hungary. [Haldrup, Kristoffer; van Driel, Tim B.; Kjaer, Kasper S.; Nielsen, Martin M.] Tech Univ Denmark, Dept Phys, Ctr Mol Movies, DK-2800 Lyngby, Denmark. [Glatzel, Pieter; Gallo, Erik; Rovezzi, Mauro] European Synchrotron Radiat Facil, F-38043 Grenoble 9, France. [March, Anne Marie; Doumy, Gilles; Young, Linda; Southworth, Stephen H.] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. [Britz, Alexander; Galler, Andreas; Assefa, Tadesse; Bressler, Christian; Gawelda, Wojciech] European XFEL, D-22761 Hamburg, Germany. [Britz, Alexander; Bressler, Christian] Hamburg Ctr Ultrafast Imaging, D-22761 Hamburg, Germany. [Cabaret, Delphine; Juhin, Amelie] Univ Paris 06, Sorbonne Univ, UMR CNRS 7590, Museum Natl Hist Nat,IMPMC,UR IRD 206, F-75005 Paris, France. [Kjaer, Kasper S.; Uhlig, Jens; Sundstrom, Villy] Lund Univ, Dept Chem Phys, S-22100 Lund, Sweden. [Dohn, Asmus; Moller, Klaus B.] Tech Univ Denmark, Dept Chem, Ctr Mol Movies, DK-2800 Lyngby, Denmark. [Lemke, Henrik T.] SLAC Natl Accelerator Lab, Linac Coherent Light Source, Menlo Pk, CA 94025 USA. [Rozgonyi, Tams] Hungarian Acad Sci, Res Ctr Nat Sci, H-1519 Budapest, Hungary. RP Vanko, G (reprint author), Hungarian Acad Sci, Wigner Res Ctr Phys, POB 49, H-1525 Budapest, Hungary. EM vanko.gyorgy@wigner.mta.hu RI Vanko, Gyorgy/B-8176-2012; Nielsen, Martin/A-5133-2009; Uhlig, Jens/A-5475-2010; Haldrup, Kristoffer/J-6875-2013; Nemeth, Zoltan/B-7037-2014; Moller, Klaus Braagaard/B-7647-2014; Dohn, Asmus/K-2808-2015; JUHIN, Amelie/C-3502-2015; Lemke, Henrik Till/N-7419-2016; Gawelda, Wojciech/B-7878-2014; Glatzel, Pieter/E-9958-2010; OI Vanko, Gyorgy/0000-0002-3095-6551; Nielsen, Martin/0000-0002-8135-434X; Uhlig, Jens/0000-0002-0528-0422; Haldrup, Kristoffer/0000-0002-0565-6397; Moller, Klaus Braagaard/0000-0002-9797-7437; JUHIN, Amelie/0000-0003-0752-3034; Lemke, Henrik Till/0000-0003-1577-8643; Gawelda, Wojciech/0000-0001-7824-9197; Glatzel, Pieter/0000-0001-6532-8144; Papai, Matyas Imre/0000-0002-4819-0611; Rovezzi, Mauro/0000-0003-2539-6198 FU European Research Council [ERC-StG-259709, ERC-AdvG-VISCHEM-226136]; 'Lendulet' (Momentum) Program of the Hungarian Academy of Sciences; European XFEL; Danish National Research Foundation's Centre for Molecular Movies; DANSCATT; Centre of Ultrafast Imaging (Hamburg); EU; Deutsche Forschungsgemeinschaft [SFB925]; French Ministry of Foreign Affairs (MAE); French Ministry of Higher Education and Research (MESR) [27875YK]; Hungarian and French Intergovernmental SAMP;T Cooperation Program [TET11FR-XTHEOEXP]; Bolyai Fellowship of the Hungarian Academy of Sciences; Knut and Alice Wallenberg Foundation; U.S. DOE [DE-AC02-06CH11357] FX This project was supported by the European Research Council via contracts ERC-StG-259709 and ERC-AdvG-VISCHEM-226136, the 'Lendulet' (Momentum) Program of the Hungarian Academy of Sciences, and the European XFEL. K.H., M.N., T. B. van D., K.K, and H.L. acknowledge support from the Danish National Research Foundation's Centre for Molecular Movies and DANSCATT. C.B., W.G, A.G., A.B., and TA. acknowledge funding by the Centre of Ultrafast Imaging (Hamburg), by the EU-funded Cluster of Research Infrastructures for Synergies in Physics (CRISP) project, and the Deutsche Forschungsgemeinschaft via SFB925. A.B., N.Z, G.V., D.C., and A.J. acknowledge the French Ministry of Foreign Affairs (MAE) and the French Ministry of Higher Education and Research (MESR) for funding through Balaton project no. 27875YK, as well as the Hungarian and French Intergovernmental S&T Cooperation Program (TET11FR-XTHEOEXP). Z.N. acknowledges support from the Bolyai Fellowship of the Hungarian Academy of Sciences. J.U. acknowledges continued funding from the Knut and Alice Wallenberg Foundation. D.C. and A.J. acknowledge GENCI (Grand Equipement National de Calcul Intensif), which allows access to the HPC resouces of IDRIS under the allocation 2013-100172. Use of the Advanced Photon Source, an Office of Science User Facility operated for U.S. Department Of Energy Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under contract no. DE-AC02-06CH11357. We are grateful to the staff of 7-ID from the APS and the staff of ID26 from the ESRF for help during experiments. NR 76 TC 18 Z9 18 U1 5 U2 46 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAR 19 PY 2015 VL 119 IS 11 BP 5888 EP 5902 DI 10.1021/acs.jpcc.5b00557 PG 15 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CE1FP UT WOS:000351557800015 ER PT J AU Schultz, AM Brown, TD Ohodnicki, PR AF Schultz, Andrew M. Brown, Thomas D. Ohodnicki, Paul R., Jr. TI Optical and Chemi-Resistive Sensing in Extreme Environments: La-Doped SrTiO3 Films for Hydrogen Sensing at High Temperatures SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID SURFACE-PLASMON RESONANCE; THIN-FILMS; STRONTIUM-TITANATE; GAS-SENSORS; METAL-OXIDES; LANTHANUM; REDUCTION; BEHAVIOR; ZNO AB For efficient operation of next-generation fossil fuel technologies, development of sensors capable of withstanding harsh environments is required. Optical waveguide based sensing platforms have become increasingly important, but a need exists for materials that exhibit useful changes in optical properties in response to changing gas atmospheres at high temperatures. In this manuscript, the onset of a near-IR absorption associated with an increase in free carrier density in doped metal oxide films to form so-called conducting metal oxides is discussed in the context of results obtained for undoped and La-doped SrTiO3 films. Film characterization results are presented along with measured changes in optical absorption resulting from various high temperature treatments in a range of gas atmospheres. Optical property changes are also discussed in the context of a simple model for optical absorption in conducting metal oxide thin films. The combination of experimental results and theoretical modeling presented here suggests that such materials have potential for high temperature optical gas sensing applications. Simulated sensing experiments were performed at 600-800 degrees C, and a useful, rapid, and reproducible near-IR optical sensing response to H-2 confirms that this class of materials shows great promise for optical gas sensing. C1 [Schultz, Andrew M.; Brown, Thomas D.; Ohodnicki, Paul R., Jr.] Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. RP Ohodnicki, PR (reprint author), Natl Energy Technol Lab, 626 Cochrans Mill Rd, Pittsburgh, PA 15236 USA. EM paul.ohodnicki@ned.doe.gov FU U.S. DOE Advanced Research/Crosscutting Technologies program at the National Energy Technology Laboratory; U.S. Department of Energy; agency of the United States Government FX This work was funded by the U.S. DOE Advanced Research/Crosscutting Technologies program at the National Energy Technology Laboratory. This research was supported in part by an appointment to the National Energy Technology Laboratory Research Participation Program, sponsored by the U.S. Department of Energy and administered by the Oak Ridge Institute for Science and Education. This report was prepared as an account of work sponsored by an agency of the United States Government. Neither the United States Government nor any agency thereof, nor any of their employees, makes any warranty, express or implied, or assumes any legal liability or responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would not infringe privately owned rights. Reference herein to any specific commercial product, process, or service by trade name, trademark, manufacturer, or otherwise does not necessarily constitute or imply its endorsement, recommendation, or favoring by the United States Government or any agency thereof. The views and opinions of authors expressed herein do not necessarily state or reflect those of the United States Government or any agency thereof. NR 55 TC 3 Z9 3 U1 6 U2 32 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAR 19 PY 2015 VL 119 IS 11 BP 6211 EP 6220 DI 10.1021/jp512391f PG 10 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CE1FP UT WOS:000351557800050 ER PT J AU Zhang, GB Ratner, MA Reuter, MG AF Zhang, Gaibo Ratner, Mark A. Reuter, Matthew G. TI Is Molecular Rectification Caused by Asymmetric Electrode Couplings or by a Molecular Bias Drop? SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID CURRENT-VOLTAGE CHARACTERISTICS; STATISTICAL-ANALYSIS; CHARGE-TRANSPORT; CONDUCTANCE HISTOGRAMS; BREAK JUNCTIONS; ELECTRICAL CONDUCTANCE; QUANTUM INTERFERENCE; STOCHASTIC EVENTS; SINGLE; WIRES AB We investigate possible causes of molecular rectification in electrodemoleculeelectrode junctions. By using a simple model and simulated conductance histograms, we show that a molecular bias drop is responsible for rectification; conversely, asymmetric moleculeelectrode couplings do not directly result in rectification. Instead, the degree of coupling (a)symmetry can be observed in the line shapes of the conductance histograms used to experimentally assess the currentvoltage properties of such molecular junctions. More coupling asymmetry leads to less positively skewed histogram peaks. C1 [Zhang, Gaibo] Oak Ridge High Sch, Oak Ridge, TN 37830 USA. [Zhang, Gaibo; Reuter, Matthew G.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. [Reuter, Matthew G.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Ratner, Mark A.; Reuter, Matthew G.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. RP Reuter, MG (reprint author), SUNY Stony Brook, Dept Appl Math & Stat, Stony Brook, NY 11794 USA. EM matthew.reuter@stonybrook.edu OI Zhang, Gaibo/0000-0002-0823-1829 FU Eugene P. Wigner Fellowship while at the Oak Ridge National Laboratory; U.S. Department of Energy [DE-AC05-00OR22725]; U.S. Air Force Office of Scientific Research Multidisciplinary University Research Initiative [FA9550-14-1-003] FX We thank Nongjian Tao and Latha Venkataraman for helpful conversations. G.Z. performed this research as part of a Math-Science Senior Thesis at the Oak Ridge High School. M.G.R. was supported by a Eugene P. Wigner Fellowship while at the Oak Ridge National Laboratory, which is managed by UT-Battelle, LLC, for the U.S. Department of Energy under Contract DE-AC05-00OR22725. M.A.R. and M.G.R. (while at Northwestern) were supported by the U.S. Air Force Office of Scientific Research Multidisciplinary University Research Initiative (FA9550-14-1-003). The figures were prepared with the SciDraw package.74 NR 73 TC 11 Z9 11 U1 1 U2 32 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAR 19 PY 2015 VL 119 IS 11 BP 6254 EP 6260 DI 10.1021/jp5093515 PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CE1FP UT WOS:000351557800055 ER PT J AU Senty, TR Cushing, SK Wang, CJ Matranga, C Bristow, AD AF Senty, Tess R. Cushing, Scott K. Wang, Congjun Matranga, Christopher Bristow, Alan D. TI Inverting Transient Absorption Data to Determine Transfer Rates in Quantum Dot-TiO2 Heterostructures SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID ELECTRON-TRANSFER DYNAMICS; DETAILED BALANCE LIMIT; SEMICONDUCTOR NANOCRYSTALS; TIO2 NANOPARTICLES; SOLAR-CELLS; CHARGE SEPARATION; CDSE NANOCRYSTALS; DOTS; RECOMBINATION; EFFICIENCY AB Transient absorption spectroscopy is a powerful technique for understanding charge carrier dynamics and recombination pathways. Analyzing the results is not trivial due to nonexponential relaxation dynamics away from equilibrium, leading to a disparity in reported charge-transfer rates. An inversion analysis technique is presented that transforms transient signals back into their original rate equation. The technique is demonstrated on two CdSe/TiO2 heterostructures with different surface states. Auger recombination is identified at higher carrier densities and radiative recombination at lower carrier densities. The heterostructure with additional surface traps exhibits increased trap-state Auger recombination at high carrier densities and changes to radiative recombination at low carrier densities due to a Shockley-Read-Hall process. Carrier-dependent electron-transfer rates are determined and compared to common methods that only capture the magnitude of the charge transfer at specific carrier densities. The presented transient absorption analysis provides direct understanding of the recombination mechanisms with minimal additional analysis or with presumption of decay mechanisms. C1 [Senty, Tess R.; Cushing, Scott K.; Bristow, Alan D.] W Virginia Univ, Dept Phys & Astron, Morgantown, WV 26506 USA. [Wang, Congjun; Matranga, Christopher] US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. RP Bristow, AD (reprint author), W Virginia Univ, Dept Phys & Astron, Morgantown, WV 26506 USA. EM alan.bristow@mail.wvu.edu RI Matranga, Christopher/E-4741-2015; OI Matranga, Christopher/0000-0001-7082-5938; Cushing, Scott/0000-0003-3538-2259 FU National Science Foundation [CBET-1233795]; West Virginia Higher Education Policy Commission [HEPC.dsr.12.29]; NSF Research Graduate Fellowship [GRFP-1102689] FX The authors wish to thank James P. Lewis and Oshada Ranasingha for useful discussions. The work at WVU was sponsored by the National Science Foundation (CBET-1233795) and the West Virginia Higher Education Policy Commission (HEPC.dsr.12.29). S.K.C. is supported by a NSF Research Graduate Fellowship (GRFP-1102689). We acknowledge use of the WVU Shared Research Facilities. NR 36 TC 5 Z9 5 U1 2 U2 35 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAR 19 PY 2015 VL 119 IS 11 BP 6337 EP 6343 DI 10.1021/jp512500g PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CE1FP UT WOS:000351557800064 ER PT J AU Paeng, D Lee, D Yeo, J Yoo, JH Allen, FI Kim, E So, H Park, HK Minor, AM Grigoropoulos, CP AF Paeng, Dongwoo Lee, Daeho Yeo, Junyeob Yoo, Jae-Hyuck Allen, Frances I. Kim, Eunpa So, Hongyun Park, Hee K. Minor, Andrew M. Grigoropoulos, Costas P. TI Laser-Induced Reductive Sintering of Nickel Oxide Nanoparticles under Ambient Conditions SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID NIO THIN-FILMS; PRINTED ELECTRONICS; NO2 GAS; SUPERCAPACITOR; TEMPERATURE; NANOSTRUCTURES; PERFORMANCE; FABRICATION; MECHANISM; ARRAYS AB This work is concerned with the kinetics of laser-induced reductive sintering of nonstoichiometric crystalline nickel oxide (NiO) nanoparticles (NPs) under ambient conditions. The mechanism of photophysical reductive sintering upon irradiation using a 514.5 nm continuous-wave (CW) laser on NiO NP thin films has been studied through modulating the laser power density and illumination time. Protons produced due to high-temperature decomposition of the solvent present in the NiO NP ink, oxygen vacancies in the NiO NPs, and electronic excitation in the NiO NPs by laser irradiation all affect the early stage of the reductive sintering process. Once NiO NPs are reduced by laser irradiation to Ni, they begin to coalesce, forming a conducting material. In situ optical and electrical measurements during the reductive sintering process take advantage of the distinct differences between the oxide and the metallic phases to monitor the transient evolution of the process. We observe four regimes: oxidation, reduction, sintering, and reoxidation. A characteristic time scale is assigned to each regime. C1 [Paeng, Dongwoo; Yeo, Junyeob; Yoo, Jae-Hyuck; Kim, Eunpa; So, Hongyun; Grigoropoulos, Costas P.] Univ Calif Berkeley, Dept Mech Engn, Berkeley, CA 94720 USA. [Lee, Daeho] Gachon Univ, Dept Mech Engn, Songnam 461701, Gyeonggi Do, South Korea. [Allen, Frances I.; Minor, Andrew M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Natl Ctr Electron Microscopy, Berkeley, CA 94720 USA. [Allen, Frances I.; Minor, Andrew M.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Park, Hee K.] Laser Prismat LLC, San Jose, CA 95129 USA. RP Grigoropoulos, CP (reprint author), Univ Calif Berkeley, Dept Mech Engn, Berkeley, CA 94720 USA. EM cgrigoro@berkeley.edu RI Foundry, Molecular/G-9968-2014; Yeo, Junyeob/I-1287-2013; OI Yeo, Junyeob/0000-0001-7422-3467; Lee, Daeho/0000-0002-8119-9677 FU King Abdullah University of Science and Technology (KAUST); SBIR Phase I Grant from the U.S. National Science Foundation [1346088]; Gachon University [GCU-2014-0107]; Office of Science, Office of Basic Energy Sciences, Scientific User Facilities Division, of the U.S. Department of Energy [DE-AC02-05CH11231] FX Partial support to the Laser Thermal Laboratory by the King Abdullah University of Science and Technology (KAUST) is acknowledged. Laser Prismatics LLC was supported by the SBIR Phase I Grant No. 1346088 from the U.S. National Science Foundation. D.L. was supported by Gachon University research fund of 2014(GCU-2014-0107). The TEM analysis was performed at the Molecular Foundry, which is supported by the Office of Science, Office of Basic Energy Sciences, Scientific User Facilities Division, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The authors would also like to thank Dr. Jaewon Jang for assistance with the experiments and helpful discussions. NR 55 TC 13 Z9 13 U1 4 U2 33 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAR 19 PY 2015 VL 119 IS 11 BP 6363 EP 6372 DI 10.1021/jp512776p PG 10 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CE1FP UT WOS:000351557800067 ER PT J AU Soragni, A Yousefi, S Stoeckle, C Soriaga, AB Sawaya, MR Kozlowski, E Schmid, I Radonjic-Hoesli, S Boutet, S Williams, GJ Messerschmidt, M Seibert, MM Cascio, D Zatsepin, NA Burghammer, M Riekel, C Colletier, JP Riek, R Eisenberg, DS Simon, HU AF Soragni, Alice Yousefi, Shida Stoeckle, Christina Soriaga, Angela B. Sawaya, Michael R. Kozlowski, Evelyne Schmid, Ines Radonjic-Hoesli, Susanne Boutet, Sebastien Williams, Garth J. Messerschmidt, Marc Seibert, M. Marvin Cascio, Duilio Zatsepin, Nadia A. Burghammer, Manfred Riekel, Christian Colletier, Jacques-Philippe Riek, Roland Eisenberg, David S. Simon, Hans-Uwe TI Toxicity of Eosinophil MBP Is Repressed by Intracellular Crystallization and Promoted by Extracellular Aggregation SO MOLECULAR CELL LA English DT Article ID MAJOR BASIC-PROTEIN; GRANULE PROTEINS; ANTIMICROBIAL PEPTIDE; AMYLOID DEPOSITS; AMPHOTERICIN-B; DISEASE; FIBRILS; OLIGOMERS; MECHANISM; HEALTH AB Eosinophils are white blood cells that function in innate immunity and participate in the pathogenesis of various inflammatory and neoplastic disorders. Their secretory granules contain four cytotoxic proteins, including the eosinophil major basic protein (MBP-1). How MBP-1 toxicity is controlled within the eosinophil itself and activated upon extracellular release is unknown. Here we show how intragranular MBP-1 nanocrystals restrain toxicity, enabling its safe storage, and characterize them with an X-ray-free electron laser. Following eosinophil activation, MBP-1 toxicity is triggered by granule acidification, followed by extracellular aggregation, which mediates the damage to pathogens and host cells. Larger non-toxic amyloid plaques are also present in tissues of eosinophilic patients in a feedback mechanism that likely limits tissue damage under pathological conditions of MBP-1 oversecretion. Our results suggest that MBP-1 aggregation is important for innate immunity and immunopathology mediated by eosinophils and clarify how its polymorphic self-association pathways regulate toxicity intra-and extracellularly. C1 [Soragni, Alice; Soriaga, Angela B.; Sawaya, Michael R.; Cascio, Duilio; Eisenberg, David S.] Univ Calif Los Angeles, UCLA DOE Inst, HHMI, Los Angeles, CA 90095 USA. [Soragni, Alice; Soriaga, Angela B.; Sawaya, Michael R.; Cascio, Duilio; Eisenberg, David S.] Univ Calif Los Angeles, Dept Biol Chem, Los Angeles, CA 90095 USA. [Soragni, Alice; Soriaga, Angela B.; Sawaya, Michael R.; Cascio, Duilio; Eisenberg, David S.] Univ Calif Los Angeles, Dept Chem & Biochem, Los Angeles, CA 90095 USA. [Soragni, Alice; Yousefi, Shida; Stoeckle, Christina; Kozlowski, Evelyne; Schmid, Ines; Radonjic-Hoesli, Susanne; Simon, Hans-Uwe] Univ Bern, Inst Pharmacol, CH-3010 Bern, Switzerland. [Soragni, Alice; Riek, Roland] ETH, Dept Phys Chem, CH-8093 Zurich, Switzerland. [Boutet, Sebastien; Williams, Garth J.; Seibert, M. Marvin] SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA. [Messerschmidt, Marc] Natl Sci Fdn, BioXFEL Sci & Technol Ctr, Buffalo, NY 14203 USA. [Zatsepin, Nadia A.] Arizona State Univ, Dept Phys, Tempe, AZ 85287 USA. [Burghammer, Manfred; Riekel, Christian] European Synchrotron Radiat Facil, F-38043 Grenoble, France. [Burghammer, Manfred] Univ Ghent, Dept Analyt Chem, B-9000 Ghent, Belgium. [Colletier, Jacques-Philippe] Univ Grenoble Alpes, IBS, F-38044 Grenoble, France. [Colletier, Jacques-Philippe] CNRS, IBS, F-38044 Grenoble, France. [Colletier, Jacques-Philippe] CEA, IBS, F-38044 Grenoble, France. RP Riek, R (reprint author), ETH, Dept Phys Chem, Wolfgang Pauli Str 10, CH-8093 Zurich, Switzerland. EM roland.riek@phys.chem.ethz.ch; hus@pki.unibe.ch RI Messerschmidt, Marc/F-3796-2010; Yousefi, Shida/L-9689-2016; OI Messerschmidt, Marc/0000-0002-8641-3302; Yousefi, Shida/0000-0002-9855-4305; Simon, Hans-Uwe/0000-0002-9404-7736; Soragni, Alice/0000-0002-6634-2885 FU National Center for Research Resources [5P41RR015301-10]; National Institute of General Medical Sciences from the NIH [8 P41 GM103403-10]; DOE [DE-AC02-06CH11357]; NIH [1S10RR23057, AG029430]; CNSI at UCLA; Swiss National Science Foundation; National Science Foundation [MCB 1021557, MCB 0958111]; Allergie-Stiftung Ulrich Muller-Gierok; German Research Foundation; Keck Foundation; HHMI FX We thank all patients and collaborating clinicians for providing blood and tissue samples for the research reported here. We thank M. Capel, K. Rajashankar, N. Sukumar, J. Schuermann, I. Kourinov, and F. Murphy at NECAT beamlines 24-ID at APS, which are supported by grants from the National Center for Research Resources (5P41RR015301-10) and the National Institute of General Medical Sciences (8 P41 GM103403-10) from the NIH. Use of the APS is supported by the DOE under Contract DE-AC02-06CH11357. We thank Matthias Frank, Mark S. Hunter, Michael J. Bogan, and John Miao for helpful experimental suggestions and scientific discussion; Anton Barty for help with XFEL image conversion and preliminary data analysis; and Stephan Stern and Tom Pardini for helping with the XFEL motor script. We thank the ESRF and LCLS staff for technical support. We acknowledge the EMEZ facility at ETH for support with the electron microscopy experiments, in particular Elisabeth Gruber-Miller, Fabian Gramm, and Peter Tittmann. We also acknowledge the use of instruments at the Electron Imaging Center for NanoMachines supported by NIH (1S10RR23057) and CNSI at UCLA. This work was supported by grants from the Swiss National Science Foundation (to R.R. and H.-U.S.); the National Science Foundation (MCB 1021557 to N.A.Z. and MCB 0958111 to D.S.E.); the Allergie-Stiftung Ulrich Muller-Gierok (to S.R.-H. and H.-U.S.); the German Research Foundation (to C.S.); and from the NIH (AG029430), the Keck Foundation, and HHMI (to D.S.E.). NR 55 TC 16 Z9 16 U1 2 U2 9 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 1097-2765 EI 1097-4164 J9 MOL CELL JI Mol. Cell PD MAR 19 PY 2015 VL 57 IS 6 BP 1011 EP 1021 DI 10.1016/j.molcel.2015.01.026 PG 11 WC Biochemistry & Molecular Biology; Cell Biology SC Biochemistry & Molecular Biology; Cell Biology GA CE3GP UT WOS:000351715000009 PM 25728769 ER PT J AU Lee, N Schuck, PJ Nico, PS Gilbert, B AF Lee, Namhey Schuck, P. James Nico, Peter S. Gilbert, Benjamin TI Surface Enhanced Raman Spectroscopy of Organic Molecules on Magnetite (Fe3O4) Nanoparticles SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID DOPED SEMICONDUCTOR NANOCRYSTALS; SITU ATR-FTIR; OXALATE ADSORPTION; OXIDE NANOCRYSTALS; AMINO-ACIDS; HEMATITE; COMPLEXATION; CYSTEINE; SILVER; TIO2 AB Surface-enhanced Raman spectroscopy (SERS) of species bound to environmentally relevant oxide nanoparticles is largely limited to organic molecules structurally related to catechol that facilitate a chemical enhancement of the Raman signal. Here, we report that magnetite (Fe3O4) nanoparticles provide a SERS signal from oxalic acid and cysteine via an electric field enhancement Magnetite thus likely provides an oxide substrate for SERS study of any adsorbed organic molecule. This substrate combines benefits from both metal-based and chemical SERS by providing an oxide surface for studies of environmentally and catalytically relevant detailed chemical bonding information with fewer restrictions of molecular structure or binding mechanisms. Therefore, the magnetite-based SERS demonstrated here provides a new approach to establishing the surface interactions of environmentally relevant organic ligands and mineral surfaces. C1 [Lee, Namhey; Nico, Peter S.; Gilbert, Benjamin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Schuck, P. James] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 91125 USA. RP Gilbert, B (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. EM bgilbert@lbl.gov RI Nico, Peter/F-6997-2010; Gilbert, Benjamin/E-3182-2010; Foundry, Molecular/G-9968-2014 OI Nico, Peter/0000-0002-4180-9397; FU Laboratory Directed Research and Development program at Berkeley Lab through the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-05CH11231]; Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231] FX The authors greatly appreciate discussions with Dr. Nicholas Borys. We thank Jennifer Soltis for acquiring TEM images of magnetite nanoparticles. We also wish to express our thanks to Patricia Fox for her assistance with ATR-FTIR data collection. This work was supported by the Laboratory Directed Research and Development program at Berkeley Lab, through the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Award Number DE-AC02-05CH11231. Work at the Molecular Foundry was supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract Number DE-AC02-05CH11231. NR 40 TC 9 Z9 9 U1 10 U2 96 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD MAR 19 PY 2015 VL 6 IS 6 BP 970 EP 974 DI 10.1021/acs.jpclett.5b00036 PG 5 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CE1HQ UT WOS:000351563100010 PM 26262854 ER PT J AU May, KJ Fenning, DP Ming, T Hong, WT Lee, D Stoerzinger, KA Biegalski, MD Kolpak, AM Shao-Horn, Y AF May, Kevin J. Fenning, David P. Ming, Tian Hong, Wesley T. Lee, Dongkyu Stoerzinger, Kelsey A. Biegalski, Michael D. Kolpak, Alexie M. Shao-Horn, Yang TI Thickness-Dependent Photoelectrochemical Water Splitting on Ultrathin LaFeO3 Films Grown on Nb:SrTiO3 SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID CURRENT-VOLTAGE CHARACTERISTICS; P-N-JUNCTION; SEMICONDUCTOR ELECTRODES; ADVENTITIOUS CARBON; BAND OFFSETS; SOLAR-CELLS; PEROVSKITE; HETEROJUNCTION; EVOLUTION; STATES AB The performance of photoelectrodes can be modified by changing the material chemistry, geometry, and interface engineering. Specifically, nanoscale active layers can facilitate the collection of charge carriers. In heterostructure devices, the multiple material interfaces are particularly important, which at present are not well understood for oxides. Here, we report a detailed study of ultrathin (2-25 nm) LaFeO3 films grown epitaxially on Nb-doped SrTiO3. The films exhibit thickness-dependence with sensitivity to less than 10 nm in both the through-plane charge transfer conductivity and in the potential-dependent photoresponse. Supplementing photoelectrochemical measurements with X-ray photoelectron spectroscopy, spectroscopic ellipsometry, and electrochemical impedance spectroscopy, we construct a band model that accounts for this thickness dependence via a shifting valence-band offset at the film-substrate interface and the potential-dependent overlap of the depletion regions present at both the film-substrate and film-electrolyte interfaces. These results illustrate the utility of using active layer thickness and film-substrate interactions to tune the performance of photoelectrodes, providing insight for the design of efficient heterostructure oxide photoelectrochemical devices. C1 [May, Kevin J.; Fenning, David P.; Lee, Dongkyu; Kolpak, Alexie M.; Shao-Horn, Yang] MIT, Dept Mech Engn, Cambridge, MA 02139 USA. [Ming, Tian; Hong, Wesley T.; Stoerzinger, Kelsey A.; Shao-Horn, Yang] MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA. [Shao-Horn, Yang] MIT, Electrochem Energy Lab, Cambridge, MA 02139 USA. [Biegalski, Michael D.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP May, KJ (reprint author), MIT, Dept Mech Engn, Cambridge, MA 02139 USA. EM kjmay@alum.mit.edu; dfenning@eng.ucsd.edu; shaohorn@mit.edu OI May, Kevin/0000-0002-1082-8333; Stoerzinger, Kelsey/0000-0002-3431-8290 FU Natural Sciences and Engineering Research Council of Canada (NSERC); MIT/Battelle postdoctoral associate program; National Science Foundation Graduate Research Fellowship [DGE-1122374]; MRSEC Program of the National Science Foundation [DMR-0819762]; King Fahd University of Petroleum and Minerals in Dharam, Saudi Arabia through the Center for Clean Water and Clean Energy at MIT and KFUPM; National Science Foundation under NSF [ECS-0335765]; Center for Nanophase Materials Sciences FX We thank Dr. Hans Christen for helpful comments and suggestions during the preparation of this manuscript. K.J.M. was supported in part by a doctoral postgraduate scholarship (PGS-D) from the Natural Sciences and Engineering Research Council of Canada (NSERC). D.P.F. acknowledges the support of the MIT/Battelle postdoctoral associate program. K.A.S. was supported by the National Science Foundation Graduate Research Fellowship under Grant No. DGE-1122374. This work was supported in part by the MRSEC Program of the National Science Foundation under Award No. DMR-0819762, and we thank the King Fahd University of Petroleum and Minerals in Dharam, Saudi Arabia, for funding the research reported in this paper through the Center for Clean Water and Clean Energy at MIT and KFUPM. This work was performed in part at Harvard University's Center for Nanoscale Systems (CNS), a member of the National Nanotechnology Infrastructure Network (NNIN), which is supported by the National Science Foundation under NSF Award No. ECS-0335765, and in part at the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. The authors dedicate this paper to the memory of Mike Biegalski, who will be remembered for his friendship and his tireless support. NR 58 TC 10 Z9 10 U1 12 U2 120 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD MAR 19 PY 2015 VL 6 IS 6 BP 977 EP 985 DI 10.1021/acs.jpclett.5b00169 PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CE1HQ UT WOS:000351563100012 PM 26262856 ER PT J AU Jackson, NE Savoie, BM Chen, LX Ratner, MA AF Jackson, Nicholas E. Savoie, Brett M. Chen, Lin X. Ratner, Mark A. TI A Simple Index for Characterizing Charge Transport in Molecular Materials SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID ORGANIC PHOTOVOLTAICS; RESISTANCE-DISTANCE; SOLAR-CELLS; SEMICONDUCTORS; CHEMISTRY AB While advances in quantum chemistry have rendered the accurate prediction of band alignment relatively straightforward, the ability to forecast a noncrystalline, multimolecule system's conductivity possesses no simple computational form. Adapting the theory of classical resistor networks, we develop an index for quantifying charge transport in bulk molecular materials, without the requirement of crystallinity. The basic behavior of this index is illustrated through its application to simple lattices and clusters of common organic photovoltaic molecules, where it is shown to reproduce experimentally known performances for these materials. This development provides a quantitative computational means for determining a priori the bulk charge transport properties of molecular materials. C1 [Jackson, Nicholas E.; Savoie, Brett M.; Chen, Lin X.; Ratner, Mark A.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Chen, Lin X.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Ratner, MA (reprint author), Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. EM ratner@northwestern.edu FU U.S. DOE-BES Argonne-Northwestern Solar Energy Research Center (ANSER); Energy Frontier Research Center [DE-SC0001059]; NSF [NSF DGE-0824162] FX We thank the U.S. DOE-BES Argonne-Northwestern Solar Energy Research Center (ANSER), and Energy Frontier Research Center (Award DE-SC0001059) for funding this project. N.E.J. thanks the NSF for the award of a Graduate Research Fellowship (NSF DGE-0824162). NR 22 TC 10 Z9 10 U1 4 U2 23 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD MAR 19 PY 2015 VL 6 IS 6 BP 1018 EP 1021 DI 10.1021/acs.jpclett.5b00135 PG 4 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CE1HQ UT WOS:000351563100018 PM 26262862 ER PT J AU Baghani, E O'Leary, SK Fedin, I Talapin, DV Pelton, M AF Baghani, Erfan O'Leary, Stephen K. Fedin, Igor Talapin, Dmitri V. Pelton, Matthew TI Auger-Limited Carrier Recombination and Relaxation in CdSe Colloidal Quantum Wells SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID ELECTRONIC-STRUCTURE; SEMICONDUCTOR NANOPLATELETS; STIMULATED-EMISSION; DOTS; DYNAMICS; RODS AB Using time-resolved photoluminescence spectroscopy, we show that two-exciton Auger recombination dominates carrier recombination and cooling dynamics in CdSe nanoplatelets, or colloidal quantum wells. The electron hole recombination rate depends only on the number of electron hole pairs present in each nanoplatelet, and is consistent with a two-exciton recombination process over a wide range of exciton densities. The carrier relaxation rate within the conduction and valence bands also depends only on the number of electron hole pairs present, apart from an initial rapid decay, and is consistent with the cooling rate being limited by reheating due to Auger recombination processes. These Auger limited recombination and relaxation dynamics are qualitatively different from the carrier dynamics in either colloidal quantum dots or epitaxial quantum wells. C1 [Baghani, Erfan; O'Leary, Stephen K.] Univ British Columbia, Sch Engn, Kelowna, BC V1V 1V7, Canada. [Fedin, Igor; Talapin, Dmitri V.] Univ Chicago, Dept Chem, Chicago, IL 60637 USA. [Fedin, Igor; Talapin, Dmitri V.] Univ Chicago, James Franck Inst, Chicago, IL 60637 USA. [Talapin, Dmitri V.; Pelton, Matthew] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Pelton, Matthew] Univ Maryland Baltimore Cty, Dept Phys, Baltimore, MD 21250 USA. RP Pelton, M (reprint author), Argonne Natl Lab, Ctr Nanoscale Mat, 9700 S Cass Ave, Argonne, IL 60439 USA. EM mpelton@umbc.edu RI Pelton, Matthew/H-7482-2013 OI Pelton, Matthew/0000-0002-6370-8765 FU Center for Nanoscale Materials, a U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility [DE-AC02-06CH11357]; Natural Sciences and Engineering Research Council of Canada; Air Force Office of Scientific Research [FA9550-14-1-0367]; University of Chicago NSF MRSEC Program [DMR 14-20709] FX We thank Richard Schaller for valuable assistance with the optical measurements. This work was performed, in part, at the Center for Nanoscale Materials, a U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility under Contract No. DE-AC02-06CH11357. E.B. and S.K.O. gratefully acknowledge financial support from the Natural Sciences and Engineering Research Council of Canada. D.V.T. acknowledges support by the Air Force Office of Scientific Research under grant number FA9550-14-1-0367. This work used facilities supported by the University of Chicago NSF MRSEC Program under Award Number DMR 14-20709. NR 29 TC 11 Z9 11 U1 3 U2 37 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD MAR 19 PY 2015 VL 6 IS 6 BP 1032 EP 1036 DI 10.1021/acs.jpclett.5b00143 PG 5 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CE1HQ UT WOS:000351563100021 PM 26262865 ER PT J AU Zawadzki, P Zakutayev, A Lany, S AF Zawadzki, Pawel Zakutayev, Andriy Lany, Stephan TI Entropy-Driven Clustering in Tetrahedrally Bonded Multinary Materials SO PHYSICAL REVIEW APPLIED LA English DT Article ID FILM SOLAR-CELLS; KESTERITE; CU2ZNSNS4 AB Compositional inhomogeneities in multielemental materials typically form due to lowering of the energy relative to the homogeneous phase. Here, we demonstrate an entropy-driven mechanism in the zinc-blende derived cation-substituted multinary compounds Cu2SnS3 (CTS) and Cu2ZnSnS4 (CZTS). Using a motifbased model Hamiltonian and Monte Carlo simulations, we find that disorder leads to a redistribution of the structural motifs in such a way to create cation clustering. The associated formation of (sub-) nanometerscale compositional inhomogeneities can cause potential fluctuations with detrimental consequences for photovoltaic applications. C1 [Zawadzki, Pawel; Zakutayev, Andriy; Lany, Stephan] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Zawadzki, P (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM pawel.zawadzki@nrel.gov OI Zakutayev, Andriy/0000-0002-3054-5525; Lany, Stephan/0000-0002-8127-8885 FU U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, as a part of the Rapid Development of Earth-Abundant Thin Film Solar Cells [DE-AC36-08GO28308] FX This work was funded by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, as a part of the Rapid Development of Earth-Abundant Thin Film Solar Cells agreement under Contract No. DE-AC36-08GO28308 to the National Renewable Energy Laboratory (NREL). This work used computational resources sponsored by the Department of Energy's Office of Energy Efficiency and Renewable Energy, located at NREL. NR 41 TC 18 Z9 18 U1 4 U2 31 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2331-7019 J9 PHYS REV APPL JI Phys. Rev. Appl. PD MAR 19 PY 2015 VL 3 IS 3 AR 034007 DI 10.1103/PhysRevApplied.3.034007 PG 7 WC Physics, Applied SC Physics GA CD9PY UT WOS:000351431500001 ER PT J AU Singer, A Marsh, MJ Dietze, SH Uhlir, V Li, Y Walko, DA Dufresne, EM Srajer, G Cosgriff, MP Evans, PG Fullerton, EE Shpyrko, OG AF Singer, A. Marsh, M. J. Dietze, S. H. Uhlir, V. Li, Y. Walko, D. A. Dufresne, E. M. Srajer, G. Cosgriff, M. P. Evans, P. G. Fullerton, E. E. Shpyrko, O. G. TI Condensation of collective charge ordering in chromium SO PHYSICAL REVIEW B LA English DT Article ID DENSITY-WAVE; STRAIN WAVE; SUPERCONDUCTIVITY; FILMS AB We report on the dynamics of the structural order parameter in a chromium film using synchrotron radiation in response to photoinduced ultrafast excitations. Following transient optical excitations the effective lattice temperature of the film rises close to the Neel temperature and the charge-density wave (CDW) amplitude is reduced but does not appear to ever be fully destroyed. The persistence of the CDW diffraction signal demonstrates that the CDW, if destroyed by the laser pulse, must be reestablished within the 100-ps time resolution of the synchrotron x-ray pulses. Furthermore, at all times after photoexcitation, the CDW retains its low-temperature periodicity, rather than regenerating with its high-temperature period shortly after photoexcitation. The long-term evolution shows that the CDW reverts to its ground state on a time scale of 370 +/- 40 ps. We attribute the apparent persistence of the CDW to the long-lived periodic lattice displacement in chromium. This study highlights the fundamental role of the lattice distortion and its impact on the recondensation dynamics of the charge ordered state in strongly correlated materials. C1 [Singer, A.; Marsh, M. J.; Dietze, S. H.; Shpyrko, O. G.] Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. [Uhlir, V.; Fullerton, E. E.] Univ Calif San Diego, Ctr Magnet Recording Res, La Jolla, CA 92093 USA. [Li, Y.; Walko, D. A.; Dufresne, E. M.; Srajer, G.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Cosgriff, M. P.; Evans, P. G.] Univ Wisconsin, Dept Mat Sci & Engn, Madison, WI 53706 USA. RP Singer, A (reprint author), Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. EM ansinger@ucsd.edu RI Uhlir, Vojtech/E-6860-2011; Singer, Andrej/M-3948-2015; Fullerton, Eric/H-8445-2013 OI Fullerton, Eric/0000-0002-4725-9509 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001805, DE-SC0003678, DE-FG02-04ER46147]; U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory [DE-AC02-06CH11357] FX We acknowledge the help of J. Wingert, J. Stanley, and T. Saerbeck in measuring the expansion coefficient of Cr and fruitful discussions with I. A. Vartanyants. The work at UCSD was supported by U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-SC0001805 and DE-SC0003678. P.G.E. and M.P.C. acknowledge support from the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Contract No. DE-FG02-04ER46147. This research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. NR 35 TC 4 Z9 4 U1 4 U2 25 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAR 19 PY 2015 VL 91 IS 11 AR 115134 DI 10.1103/PhysRevB.91.115134 PG 8 WC Physics, Condensed Matter SC Physics GA CD9OA UT WOS:000351426500001 ER PT J AU Stollenwerk, AJ Hurley, N Beck, B Spurgeon, K Kidd, TE Gu, G AF Stollenwerk, A. J. Hurley, N. Beck, B. Spurgeon, K. Kidd, T. E. Gu, G. TI Manipulation of subsurface carbon nanoparticles in Bi2Sr2CaCu2O8+delta using a scanning tunneling microscope SO PHYSICAL REVIEW B LA English DT Article ID ELECTRONIC-PROPERTIES; NANOMETER-SCALE; SINGLE-CRYSTALS; ATOMIC-SCALE; SURFACE; STM; SUPERCONDUCTORS; NANOINDENTATION; NANOSTRUCTURES; SPECTROSCOPY AB We present evidence that subsurface carbon nanoparticles in Bi2Sr2CaCu2O8+delta can be manipulated with nanometer precision using a scanning tunneling microscope. High-resolution images indicate that most of the carbon particles remain subsurface after transport observable as a local increase in height as the particle pushes up on the surface. Tunneling spectra in the vicinity of these protrusions exhibit semiconducting characteristics with a band gap of approximately 1.8 eV, indicating that the incorporation of carbon locally alters the electronic properties near the surface. C1 [Stollenwerk, A. J.; Hurley, N.; Beck, B.; Spurgeon, K.; Kidd, T. E.] Univ No Iowa, Dept Phys, Cedar Falls, IA 50614 USA. [Gu, G.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RP Stollenwerk, AJ (reprint author), Univ No Iowa, Dept Phys, 215 Begeman Hall, Cedar Falls, IA 50614 USA. EM andrew.stollenwerk@uni.edu FU National Science Foundation [DMR-1206530, DMR-1410496]; Iowa NASA EPSCoR [NNX09AO66A]; American Chemical Society Petroleum Research Fund [53401-UNI10]; University of Northern Iowa; Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, U.S. Department of Energy [DE-AC02- 98CH10886] FX This work was supported in part by the National Science Foundation, Grants No. DMR-1206530 and No. DMR-1410496. T.E.K. and R.H. acknowledge support from Iowa NASA EPSCoR under Grant No. NNX09AO66A. R.H. also acknowledges support from the American Chemical Society Petroleum Research Fund, Grant No. 53401-UNI10. A pre-tenure summer fellowship for A.J.S. and R.H. was made available through the University of Northern Iowa. Work at Brookhaven is supported by the Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, U.S. Department of Energy, under Contract No. DE-AC02- 98CH10886. The authors thank B. Adams for useful discussions. NR 28 TC 0 Z9 0 U1 2 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAR 19 PY 2015 VL 91 IS 12 AR 125425 DI 10.1103/PhysRevB.91.125425 PG 5 WC Physics, Condensed Matter SC Physics GA CD9OC UT WOS:000351426700002 ER PT J AU Bass, M Bishai, M Cherdack, D Diwan, M Djurcic, Z Hernandez, J Lundberg, B Paolone, V Qian, X Rameika, R Whitehead, L Wilson, RJ Worcester, E Zeller, G AF Bass, M. Bishai, M. Cherdack, D. Diwan, M. Djurcic, Z. Hernandez, J. Lundberg, B. Paolone, V. Qian, X. Rameika, R. Whitehead, L. Wilson, R. J. Worcester, E. Zeller, G. TI Baseline optimization for the measurement of CP violation, mass hierarchy, and theta(23) octant in a long-baseline neutrino oscillation experiment SO PHYSICAL REVIEW D LA English DT Article ID LIQUID ARGON TPC; EXPERIMENT-SIMULATOR; MATTER AB Next-generation long-baseline electron neutrino appearance experiments will seek to discover CP violation, determine the mass hierarchy and resolve the theta(23) octant. In light of the recent precision measurements of theta(13), we consider the sensitivity of these measurements in a study to determine the optimal baseline, including practical considerations regarding beam and detector performance. We conclude that a detector at a baseline of at least 1000 km in a wide-band muon neutrino beam is the optimal configuration. C1 [Djurcic, Z.] Argonne Natl Lab, Argonne, IL 60439 USA. [Bishai, M.; Diwan, M.; Qian, X.; Worcester, E.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Bass, M.; Cherdack, D.; Wilson, R. J.] Colorado State Univ, Ft Collins, CO 80523 USA. [Lundberg, B.; Rameika, R.; Zeller, G.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Hernandez, J.; Whitehead, L.] Univ Houston, Houston, TX 77204 USA. [Paolone, V.] Univ Pittsburgh, Pittsburgh, PA 15260 USA. RP Bass, M (reprint author), Colorado State Univ, Ft Collins, CO 80523 USA. OI Qian, Xin/0000-0002-7903-7935; Wilson, Robert/0000-0002-8184-4103 FU U.S. Department of Energy, Office of Science, Office of High Energy Physics FX We would like to thank Josh Klein, William Louis, Alberto Marchionni, and Michael Mooney for their careful reading and helpful suggestions during the preparation of this manuscript. This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of High Energy Physics. NR 35 TC 18 Z9 18 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD MAR 19 PY 2015 VL 91 IS 5 AR 052015 DI 10.1103/PhysRevD.91.052015 PG 19 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CD9ON UT WOS:000351427800002 ER PT J AU Pisano, S Biselli, A Niccolai, S Seder, E Guidal, M Mirazita, M Adhikari, KP Adikaram, D Amaryan, MJ Anderson, MD Pereira, SA Avakian, H Ball, J Battaglieri, M Batourine, V Bedlinskiy, I Bosted, P Briscoe, B Brock, J Brooks, WK Burkert, VD Carlin, C Carman, DS Celentano, A Chandavar, S Charles, G Colaneri, L Cole, PL Compton, N Contalbrigo, M Cortes, O Crabb, DG Crede, V D'Angelo, A De Vita, R De Sanctis, E Deur, A Djalali, C Dupre, R Egiyan, H El Alaoui, A El Fassi, L Elouadrhiri, L Eugenio, P Fedotov, G Fegan, S Fersch, R Filippi, A Fleming, JA Fradi, A Garillon, B Garcon, M Ghandilyan, Y Gilfoyle, GP Giovanetti, KL Girod, FX Goetz, JT Gohn, W Golovatch, E Gothe, RW Griffioen, KA Guo, L Hafidi, K Hanretty, C Hattawy, M Hicks, K Holtrop, M Hughes, SM Ilieva, Y Ireland, DG Ishkhanov, BS Jenkins, D Jiang, X Jo, HS Joo, K Joosten, S Keith, CD Keller, D Kim, A Kim, W Klein, FJ Kubarovsky, V Kuhn, SE Lenisa, P Livingston, K Lu, HY MacCormick, M MacGregor, IJD Mayer, M McKinnon, B Meekins, DG Meyer, CA Mokeev, V Montgomery, RA Moody, CI Camacho, CM Nadel-Turonski, P Osipenko, M Ostrovidov, AI Park, K Phelps, W Phillips, JJ Pogorelko, O Price, JW Procureur, S Prok, Y Puckett, AJR Ripani, M Rizzo, A Rosner, G Rossi, P Roy, P Sabatie, F Salgado, C Schott, D Schumacher, RA Skorodumina, I Smith, GD Sober, DI Sokhan, D Sparveris, N Stepanyan, S Stoler, P Strauch, S Sytnik, V Tian, Y Tkachenko, S Turisini, M Ungaro, M Voutier, E Walford, NK Watts, DP Wei, X Weinstein, LB Wood, MH Zachariou, N Zana, L Zhang, J Zhao, ZW Zonta, I AF Pisano, S. Biselli, A. Niccolai, S. Seder, E. Guidal, M. Mirazita, M. Adhikari, K. P. Adikaram, D. Amaryan, M. J. Anderson, M. D. Pereira, S. Anefalos Avakian, H. Ball, J. Battaglieri, M. Batourine, V. Bedlinskiy, I. Bosted, P. Briscoe, B. Brock, J. Brooks, W. K. Burkert, V. D. Carlin, C. Carman, D. S. Celentano, A. Chandavar, S. Charles, G. Colaneri, L. Cole, P. L. Compton, N. Contalbrigo, M. Cortes, O. Crabb, D. G. Crede, V. D'Angelo, A. De Vita, R. De Sanctis, E. Deur, A. Djalali, C. Dupre, R. Egiyan, H. El Alaoui, A. El Fassi, L. Elouadrhiri, L. Eugenio, P. Fedotov, G. Fegan, S. Fersch, R. Filippi, A. Fleming, J. A. Fradi, A. Garillon, B. Garcon, M. Ghandilyan, Y. Gilfoyle, G. P. Giovanetti, K. L. Girod, F. X. Goetz, J. T. Gohn, W. Golovatch, E. Gothe, R. W. Griffioen, K. A. Guo, L. Hafidi, K. Hanretty, C. Hattawy, M. Hicks, K. Holtrop, M. Hughes, S. M. Ilieva, Y. Ireland, D. G. Ishkhanov, B. S. Jenkins, D. Jiang, X. Jo, H. S. Joo, K. Joosten, S. Keith, C. D. Keller, D. Kim, A. Kim, W. Klein, F. J. Kubarovsky, V. Kuhn, S. E. Lenisa, P. Livingston, K. Lu, H. Y. MacCormick, M. MacGregor, I. J. D. Mayer, M. McKinnon, B. Meekins, D. G. Meyer, C. A. Mokeev, V. Montgomery, R. A. Moody, C. I. Camacho, C. Munoz Nadel-Turonski, P. Osipenko, M. Ostrovidov, A. I. Park, K. Phelps, W. Phillips, J. J. Pogorelko, O. Price, J. W. Procureur, S. Prok, Y. Puckett, A. J. R. Ripani, M. Rizzo, A. Rosner, G. Rossi, P. Roy, P. Sabatie, F. Salgado, C. Schott, D. Schumacher, R. A. Skorodumina, I. Smith, G. D. Sober, D. I. Sokhan, D. Sparveris, N. Stepanyan, S. Stoler, P. Strauch, S. Sytnik, V. Tian, Ye Tkachenko, S. Turisini, M. Ungaro, M. Voutier, E. Walford, N. K. Watts, D. P. Wei, X. Weinstein, L. B. Wood, M. H. Zachariou, N. Zana, L. Zhang, J. Zhao, Z. W. Zonta, I. CA CLAS Collaboration TI Single and double spin asymmetries for deeply virtual Compton scattering measured with CLAS and a longitudinally polarized proton target SO PHYSICAL REVIEW D LA English DT Article ID GENERALIZED PARTON DISTRIBUTIONS; ELECTROPRODUCTION; NUCLEON; MESONS; QCD AB Single-beam, single-target, and double spin asymmetries for hard exclusive electroproduction of a photon on the proton (e) over right arrow(p) over right arrow. e'p'gamma are presented. The data were taken at Jefferson Lab using the CEBAF large acceptance spectrometer and a longitudinally polarized (NH3)-N-14 target. The three asymmetries were measured in 165 four-dimensional kinematic bins, covering the widest kinematic range ever explored simultaneously for beam and target-polarization observables in the valence quark region. The kinematic dependences of the obtained asymmetries are discussed and compared to the predictions of models of generalized parton distributions. The measurement of three DVCS spin observables at the same kinematic points allows a quasi-model-independent extraction of the imaginary parts of the H and (H) over tilde Compton form factors, which give insight into the electric and axial charge distributions of valence quarks in the proton. C1 [Pisano, S.; Mirazita, M.; Pereira, S. Anefalos; De Sanctis, E.; Montgomery, R. A.; Rossi, P.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Pisano, S.; Niccolai, S.; Guidal, M.; Charles, G.; Dupre, R.; Fradi, A.; Garillon, B.; Hattawy, M.; Jo, H. S.; MacCormick, M.; Camacho, C. Munoz] Inst Phys Nucl, F-91406 Orsay, France. [Biselli, A.] Fairfield Univ, Fairfield, CT 06824 USA. [Seder, E.; Gohn, W.; Joo, K.; Puckett, A. J. R.; Ungaro, M.] Univ Connecticut, Storrs, CT 06269 USA. [Seder, E.; Ball, J.; Garcon, M.; Procureur, S.] CEA, Ctr Saclay, Irfu Serv Phys Nucl, F-91191 Gif Sur Yvette, France. [Adhikari, K. P.; Amaryan, M. J.; El Fassi, L.; Kuhn, S. E.; Mayer, M.; Prok, Y.; Tkachenko, S.; Weinstein, L. B.; Zhang, J.; Zhao, Z. W.] Old Dominion Univ, Norfolk, VA 23529 USA. [Fegan, S.; Ireland, D. G.; Livingston, K.; MacGregor, I. J. D.; McKinnon, B.; Phillips, J. J.; Rosner, G.; Sokhan, D.] Univ Glasgow, Glasgow G12 8QQ, Lanark, Scotland. [Avakian, H.; Batourine, V.; Bosted, P.; Brock, J.; Burkert, V. D.; Carlin, C.; Carman, D. S.; Deur, A.; Egiyan, H.; Elouadrhiri, L.; Girod, F. X.; Guo, L.; Keith, C. D.; Kubarovsky, V.; Meekins, D. G.; Mokeev, V.; Nadel-Turonski, P.; Park, K.; Rossi, P.; Stepanyan, S.; Ungaro, M.; Wei, X.; Zhang, J.; Zhao, Z. W.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. [Battaglieri, M.; Celentano, A.; De Vita, R.; Fegan, S.; Osipenko, M.; Ripani, M.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Bedlinskiy, I.; Pogorelko, O.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Bosted, P.; Griffioen, K. A.] Coll William & Mary, Williamsburg, VA 23187 USA. [Briscoe, B.; Schott, D.] George Washington Univ, Washington, DC 20052 USA. [Brooks, W. K.; El Alaoui, A.; Sytnik, V.] Univ Tecn Federico Santa Maria, Valparaiso, Chile. [Chandavar, S.; Compton, N.; Goetz, J. T.; Hicks, K.; Keller, D.] Ohio Univ, Athens, OH 45701 USA. [Colaneri, L.; D'Angelo, A.; Rizzo, A.; Zonta, I.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, I-00133 Rome, Italy. [Colaneri, L.; D'Angelo, A.; Rizzo, A.; Zonta, I.] Univ Roma Tor Vergata, I-00133 Rome, Italy. [Cole, P. L.; Cortes, O.] Idaho State Univ, Pocatello, ID 83209 USA. [Contalbrigo, M.; Lenisa, P.; Turisini, M.] Ist Nazl Fis Nucl, Sez Ferrara, I-44100 Ferrara, Italy. [Crabb, D. G.; Hanretty, C.; Keller, D.; Prok, Y.; Tkachenko, S.] Univ Virginia, Charlottesville, VA 22901 USA. [Crede, V.; Eugenio, P.; Hanretty, C.; Ostrovidov, A. I.; Roy, P.] Florida State Univ, Tallahassee, FL 32306 USA. [Djalali, C.; Fedotov, G.; Gothe, R. W.; Ilieva, Y.; Lu, H. Y.; Park, K.; Skorodumina, I.; Strauch, S.; Tian, Ye; Wood, M. H.; Zachariou, N.; Zhao, Z. W.] Univ S Carolina, Columbia, SC 29208 USA. [Dupre, R.; El Alaoui, A.; Hafidi, K.; Moody, C. I.] Argonne Natl Lab, Argonne, IL 60439 USA. [El Alaoui, A.; Voutier, E.] Univ Grenoble Alps, CNRS IN2P3, LPSC, Grenoble, France. [Fedotov, G.; Golovatch, E.; Ishkhanov, B. S.; Mokeev, V.; Skorodumina, I.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow 119234, Russia. [Filippi, A.] Christopher Newport Univ, Newport News, VA 23606 USA. [Fleming, J. A.; Hughes, S. M.; Smith, G. D.; Sokhan, D.; Watts, D. P.; Zana, L.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Ghandilyan, Y.] Univ Edinburgh, Edinburgh EH9 3JZ, Midlothian, Scotland. [Gilfoyle, G. P.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Giovanetti, K. L.] Univ Richmond, Richmond, VA 23173 USA. [Guo, L.; Phelps, W.; Schott, D.] James Madison Univ, Harrisonburg, VA 22807 USA. [Holtrop, M.; Zana, L.] Florida Int Univ, Miami, FL 33199 USA. [Jenkins, D.] Univ New Hampshire, Durham, NH 03824 USA. [Jiang, X.] Virginia Tech, Blacksburg, VA 24061 USA. [Joosten, S.; Sparveris, N.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Kim, A.; Kim, W.] Temple Univ, Philadelphia, PA 19122 USA. [Klein, F. J.; Nadel-Turonski, P.; Sober, D. I.; Walford, N. K.] Kyungpook Natl Univ, Taegu 702701, South Korea. [Meyer, C. A.; Schumacher, R. A.] Catholic Univ Amer, Washington, DC 20064 USA. [Price, J. W.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Salgado, C.] Calif State Univ Dominguez Hills, Carson, CA 90747 USA. [Stoler, P.] Norfolk State Univ, Norfolk, VA 23504 USA. [Stoler, P.] Rensselaer Polytech Inst, Troy, NY 12180 USA. [Wood, M. H.] Canisius Coll, Buffalo, NY 14208 USA. RP Pisano, S (reprint author), Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. EM pisanos@jlab.org RI Brooks, William/C-8636-2013; Meyer, Curtis/L-3488-2014; El Alaoui, Ahmed/B-4638-2015; MacGregor, Ian/D-4072-2011; Sabatie, Franck/K-9066-2015; Schumacher, Reinhard/K-6455-2013; Osipenko, Mikhail/N-8292-2015; Zhang, Jixie/A-1461-2016; Adikaram, Dasuni/D-1539-2016; Adikaram, D/H-7128-2016; Celentano, Andrea/J-6190-2012; D'Angelo, Annalisa/A-2439-2012 OI Brooks, William/0000-0001-6161-3570; Zonta, Irene/0000-0003-4952-2160; Meyer, Curtis/0000-0001-7599-3973; Sabatie, Franck/0000-0001-7031-3975; Schumacher, Reinhard/0000-0002-3860-1827; Osipenko, Mikhail/0000-0001-9618-3013; Celentano, Andrea/0000-0002-7104-2983; D'Angelo, Annalisa/0000-0003-3050-4907 FU U.S. Department of Energy [DE-FG02-96ER40950, DE-AC05-06OR23177]; National Science Foundation; French Centre National de la Recherche Scientifique and Commissariat a l'Energie Atomique; French-American Cultural Exchange (FACE); Italian Istituto Nazionale di Fisica Nucleare; Chilean Comision Nacional de Investigacion Cientifica y Tecnologica (CONICYT); National Research Foundation of Korea; UK Science and Technology Facilities Council (STFC) FX We thank the staff of the Accelerator and the Physics Divisions and of the Target Group at Jefferson Lab for making the experiment possible. Special thanks to M. Guidal, F. Sabatie, S. Liuti, D. Muller and K. Kumericki for the theoretical support. This work was supported in part by the U.S. Department of Energy (No. DE-FG02-96ER40950) and National Science Foundation, the French Centre National de la Recherche Scientifique and Commissariat a l'Energie Atomique, the French-American Cultural Exchange (FACE), the Italian Istituto Nazionale di Fisica Nucleare, the Chilean Comision Nacional de Investigacion Cientifica y Tecnologica (CONICYT), the National Research Foundation of Korea, and the UK Science and Technology Facilities Council (STFC). The Jefferson Science Associates (JSA) operates the Thomas Jefferson National Accelerator Facility for the U.S. Department of Energy under Contract No. DE-AC05-06OR23177. NR 40 TC 13 Z9 13 U1 1 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD MAR 19 PY 2015 VL 91 IS 5 AR 052014 DI 10.1103/PhysRevD.91.052014 PG 27 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CD9ON UT WOS:000351427800001 ER PT J AU Yook, Y Kwon, YJ Abdesselam, A Adachi, I Al Said, S Arinstein, K Asner, DM Aulchenko, V Aushev, T Ayad, R Bahinipati, S Bakich, AM Bala, A Bansal, V Bhardwaj, V Bhuyan, B Bondar, A Bonvicini, G Bozek, A Bracko, M Browder, TE Cervenkov, D Chekelian, V Chen, A Cheon, BG Chilikin, K Chistov, R Cho, K Chobanova, V Choi, Y Dolezal, Z Drasal, Z Drutskoy, A Dutta, D Dutta, K Eidelman, S Farhat, H Fast, JE Ferber, T Frost, O Gaur, V Gabyshev, N Ganguly, S Garmash, A Gillard, R Glattauer, R Goh, YM Golob, B Grzymkowska, O Haba, J Hara, K Hayasaka, K Hayashii, H He, XH Heck, M Higuchi, T Horii, Y Hoshi, Y Hou, WS Iijima, T Ishikawa, A Itoh, R Iwasaki, Y Iwashita, T Jaegle, I Julius, T Kato, E Katrenko, P Kawasaki, T Kiesling, C Kim, DY Kim, JB Kim, JH Kim, KT Kim, MJ Kim, YJ Kinoshita, K Klucar, J Ko, BR Kodys, P Korpar, S Krizan, P Krokovny, P Kuhr, T Kuzmin, A Lange, JS Li, Y Gioi, LL Liu, C Liu, Y Liventsev, D Lukin, P Miyabayashi, K Miyata, H Mohanty, GB Moll, A Mussa, R Nagasaka, Y Nakamura, I Nakano, E Nakao, M Natkaniec, Z Nayak, M Nedelkovska, E Nisar, NK Nishida, S Nitoh, O Ogawa, S Okuno, S Pakhlov, P Park, CS Park, H Park, HK Pedlar, TK Pestotnik, R Petric, M Piilonen, LE Ritter, M Rohrken, M Rostomyan, A Ryu, S Saito, T Sakai, Y Sandilya, S Santelj, L Sanuki, T Sato, Y Savinov, V Schneider, O Schnell, G Schwanda, C Senyo, K Seon, O Sevior, ME Shebalin, V Shen, CP Shibata, TA Shiu, JG Shwartz, B Sibidanov, A Simon, F Sohn, YS Sokolov, A Solovieva, E Staric, M Steder, M Sumihama, M Sumiyoshi, T Tatishvili, G Teramoto, Y Trabelsi, K Uchida, M Uglov, T Urquijo, P Usov, Y Van Hulse, C Vanhoefer, P Varner, G Varvell, KE Vinokurova, A Vorobyev, V Wagner, MN Wang, CH Wang, MZ Wang, P Wang, XL Watanabe, M Watanabe, Y Wehle, S Williams, KM Won, E Yamashita, Y Yashchenko, S Yusa, Y Zhang, ZP Zhilich, V Zupanc, A AF Yook, Y. Kwon, Y. -J. Abdesselam, A. Adachi, I. Al Said, S. Arinstein, K. Asner, D. M. Aulchenko, V. Aushev, T. Ayad, R. Bahinipati, S. Bakich, A. M. Bala, A. Bansal, V. Bhardwaj, V. Bhuyan, B. Bondar, A. Bonvicini, G. Bozek, A. Bracko, M. Browder, T. E. Cervenkov, D. Chekelian, V. Chen, A. Cheon, B. G. Chilikin, K. Chistov, R. Cho, K. Chobanova, V. Choi, Y. Dolezal, Z. Drasal, Z. Drutskoy, A. Dutta, D. Dutta, K. Eidelman, S. Farhat, H. Fast, J. E. Ferber, T. Frost, O. Gaur, V. Gabyshev, N. Ganguly, S. Garmash, A. Gillard, R. Glattauer, R. Goh, Y. M. Golob, B. Grzymkowska, O. Haba, J. Hara, K. Hayasaka, K. Hayashii, H. He, X. H. Heck, M. Higuchi, T. Horii, Y. Hoshi, Y. Hou, W. -S. Iijima, T. Ishikawa, A. Itoh, R. Iwasaki, Y. Iwashita, T. Jaegle, I. Julius, T. Kato, E. Katrenko, P. Kawasaki, T. Kiesling, C. Kim, D. Y. Kim, J. B. Kim, J. H. Kim, K. T. Kim, M. J. Kim, Y. J. Kinoshita, K. Klucar, J. Ko, B. R. Kodys, P. Korpar, S. Krizan, P. Krokovny, P. Kuhr, T. Kuzmin, A. Lange, J. S. Li, Y. Gioi, L. Li Liu, C. Liu, Y. Liventsev, D. Lukin, P. Miyabayashi, K. Miyata, H. Mohanty, G. B. Moll, A. Mussa, R. Nagasaka, Y. Nakamura, I. Nakano, E. Nakao, M. Natkaniec, Z. Nayak, M. Nedelkovska, E. Nisar, N. K. Nishida, S. Nitoh, O. Ogawa, S. Okuno, S. Pakhlov, P. Park, C. -S. Park, H. Park, H. K. Pedlar, T. K. Pestotnik, R. Petric, M. Piilonen, L. E. Ritter, M. Roehrken, M. Rostomyan, A. Ryu, S. Saito, T. Sakai, Y. Sandilya, S. Santelj, L. Sanuki, T. Sato, Y. Savinov, V. Schneider, O. Schnell, G. Schwanda, C. Senyo, K. Seon, O. Sevior, M. E. Shebalin, V. Shen, C. P. Shibata, T. -A. Shiu, J. -G. Shwartz, B. Sibidanov, A. Simon, F. Sohn, Y. -S. Sokolov, A. Solovieva, E. Staric, M. Steder, M. Sumihama, M. Sumiyoshi, T. Tatishvili, G. Teramoto, Y. Trabelsi, K. Uchida, M. Uglov, T. Urquijo, P. Usov, Y. Van Hulse, C. Vanhoefer, P. Varner, G. Varvell, K. E. Vinokurova, A. Vorobyev, V. Wagner, M. N. Wang, C. H. Wang, M. -Z. Wang, P. Wang, X. L. Watanabe, M. Watanabe, Y. Wehle, S. Williams, K. M. Won, E. Yamashita, Y. Yashchenko, S. Yusa, Y. Zhang, Z. P. Zhilich, V. Zupanc, A. CA Belle Collaboration TI Search for B+ -> e(+)nu(e) and B+ -> mu(+)nu(mu) decays using hadronic tagging SO PHYSICAL REVIEW D LA English DT Article ID LEPTONIC DECAYS; BELLE; IDENTIFICATION; VIOLATION; KEKB AB We present a search for the rare leptonic decays B+ -> e(+)nu(e) and B+ -> mu(+) nu(mu) using the full Upsilon(4S) data sample of 772 x 10(6) B (B) over bar pairs collected with the Belle detector at the KEKB asymmetric-energy e(+)e(-) collider. One of the B mesons from the Upsilon(4S) -> B (B) over bar decay is fully reconstructed in a hadronic mode, while the recoiling side is analyzed for the signal decay. We find no evidence of a signal in any of the decay modes. Upper limits of the corresponding branching fractions are determined as beta(B+ -> e(+)nu(e)) < 3.5 x 10(-6) and beta(B+ -> mu(+)nu(mu)) < 2.7 x 10(-6) at 90% confidence level. 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[Ryu, S.] Seoul Natl Univ, Seoul 151742, South Korea. [Kim, D. Y.] Soongsil Univ, Seoul 156743, South Korea. [Choi, Y.] Sungkyunkwan Univ, Suwon 440746, South Korea. [Bakich, A. M.; Sibidanov, A.; Varvell, K. E.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Gaur, V.; Mohanty, G. B.; Nisar, N. K.; Sandilya, S.] Tata Inst Fundamental Res, Bombay 400005, Maharashtra, India. [Moll, A.; Simon, F.] Tech Univ Munich, Excellence Cluster Univers, D-85748 Garching, Germany. [Ogawa, S.] Toho Univ, Funabashi, Chiba 2748510, Japan. [Hoshi, Y.] Tohoku Gakuin Univ, Tagajo, Miyagi 9858537, Japan. [Ishikawa, A.; Kato, E.; Saito, T.; Sanuki, T.; Sato, Y.] Tohoku Univ, Sendai, Miyagi 9808578, Japan. [Shibata, T. -A.; Uchida, M.] Tokyo Inst Technol, Tokyo 1528550, Japan. [Sumiyoshi, T.] Tokyo Metropolitan Univ, Tokyo 1920397, Japan. [Nitoh, O.] Tokyo Univ Agr & Technol, Tokyo 1848588, Japan. [Li, Y.; Piilonen, L. E.; Williams, K. M.] Virginia Polytech Inst & State Univ, CNP, Blacksburg, VA 24061 USA. [Bonvicini, G.; Farhat, H.; Ganguly, S.; Gillard, R.] Wayne State Univ, Detroit, MI 48202 USA. [Senyo, K.] Yamagata Univ, Yamagata 9908560, Japan. [Yook, Y.; Kwon, Y. -J.; Park, C. -S.; Sohn, Y. -S.] Yonsei Univ, Seoul 120749, South Korea. RP Yook, Y (reprint author), Yonsei Univ, Seoul 120749, South Korea. RI Solovieva, Elena/B-2449-2014; Faculty of, Sciences, KAU/E-7305-2017; Pakhlov, Pavel/K-2158-2013; Uglov, Timofey/B-2406-2014; Krokovny, Pavel/G-4421-2016; Katrenko, Petr/D-1229-2016; Chilikin, Kirill/B-4402-2014; EPFL, Physics/O-6514-2016; Chistov, Ruslan/B-4893-2014; Drutskoy, Alexey/C-8833-2016; Cervenkov, Daniel/D-2884-2017 OI Solovieva, Elena/0000-0002-5735-4059; Pakhlov, Pavel/0000-0001-7426-4824; Uglov, Timofey/0000-0002-4944-1830; Krokovny, Pavel/0000-0002-1236-4667; Katrenko, Petr/0000-0002-8808-1786; Chilikin, Kirill/0000-0001-7620-2053; Chistov, Ruslan/0000-0003-1439-8390; Drutskoy, Alexey/0000-0003-4524-0422; Cervenkov, Daniel/0000-0002-1865-741X FU Ministry of Education, Culture, Sports, Science, and Technology (MEXT) of Japan; Japan Society for the Promotion of Science (JSPS); Tau-Lepton Physics Research Center of Nagoya University; Australian Research Council; Australian Department of Industry, Innovation, Science and Research; Austrian Science Fund [P 22742-N16]; National Natural Science Foundation of China [10575109, 10775142, 10825524, 10875115, 10935008, 11175187]; Ministry of Education, Youth and Sports of the Czech Republic [LG14034]; Carl Zeiss Foundation; Deutsche Forschungsgemeinschaft; VolkswagenStiftung; Department of Science and Technology of India; Istituto Nazionale di Fisica Nucleare of Italy; WCU program of the Ministry of Education Science and Technology; National Research Foundation of Korea [2011-0029457, 2012-0008143, 2012R1A1A2008330, 2013R1A1A3007772]; BRL program under NRF [KRF-2011-0020333, KRF-2011-0021196]; Center for Korean J-PARC Users [NRF-2013K1A3A7A06056592]; BK21 Plus program; GSDC of the Korea Institute of Science and Technology Information; Polish Ministry of Science and Higher Education; National Science Center; Ministry of Education and Science of the Russian Federation; Russian Federal Agency for Atomic Energy; Slovenian Research Agency; Basque Foundation for Science (IKERBASQUE); UPV/EHU [UFI 11/55]; Swiss National Science Foundation; National Science Council; Ministry of Education of Taiwan; U.S. Department of Energy; National Science FoundationMEXT for Science Research in a Priority Area ("New Development of Flavor Physics"); JSPS for Creative Scientific Research ("Evolution of Tau-lepton Physics") FX We thank the KEKB group for the excellent operation of the accelerator; the KEK cryogenics group for the efficient operation of the solenoid; and the KEK computer group, the National Institute of Informatics, and the PNNL/EMSL computing group for valuable computing and SINET4 network support. We acknowledge support from the Ministry of Education, Culture, Sports, Science, and Technology (MEXT) of Japan, the Japan Society for the Promotion of Science (JSPS), and the Tau-Lepton Physics Research Center of Nagoya University; the Australian Research Council and the Australian Department of Industry, Innovation, Science and Research; Austrian Science Fund under Grant No. P 22742-N16; the National Natural Science Foundation of China under Contracts No. 10575109, No. 10775142, No. 10825524, No. 10875115, No. 10935008 and No. 11175187; the Ministry of Education, Youth and Sports of the Czech Republic under Contract No. LG14034; the Carl Zeiss Foundation, the Deutsche Forschungsgemeinschaft and the VolkswagenStiftung; the Department of Science and Technology of India; the Istituto Nazionale di Fisica Nucleare of Italy; the WCU program of the Ministry of Education Science and Technology, National Research Foundation of Korea Grants No. 2011-0029457, No. 2012-0008143, No. 2012R1A1A2008330, No. 2013R1A1A3007772; the BRL program under NRF Grant No. KRF-2011-0020333, No. KRF-2011-0021196, Center for Korean J-PARC Users, No. NRF-2013K1A3A7A06056592; the BK21 Plus program and the GSDC of the Korea Institute of Science and Technology Information; the Polish Ministry of Science and Higher Education and the National Science Center; the Ministry of Education and Science of the Russian Federation and the Russian Federal Agency for Atomic Energy; the Slovenian Research Agency; the Basque Foundation for Science (IKERBASQUE) and the UPV/EHU under program UFI 11/55; the Swiss National Science Foundation; the National Science Council and the Ministry of Education of Taiwan; and the U.S. Department of Energy and the National Science Foundation. This work is supported by a Grant-in-Aid from MEXT for Science Research in a Priority Area ("New Development of Flavor Physics") and from JSPS for Creative Scientific Research ("Evolution of Tau-lepton Physics"). NR 31 TC 2 Z9 2 U1 0 U2 19 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD MAR 19 PY 2015 VL 91 IS 5 AR 052016 DI 10.1103/PhysRevD.91.052016 PG 8 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CD9ON UT WOS:000351427800003 ER PT J AU Narayanan, A Watson, MD Blake, SF Bruyant, N Drigo, L Chen, YL Prabhakaran, D Yan, B Felser, C Kong, T Canfield, PC Coldea, AI AF Narayanan, A. Watson, M. D. Blake, S. F. Bruyant, N. Drigo, L. Chen, Y. L. Prabhakaran, D. Yan, B. Felser, C. Kong, T. Canfield, P. C. Coldea, A. I. TI Linear Magnetoresistance Caused by Mobility Fluctuations in n-Doped Cd3As2 SO PHYSICAL REVIEW LETTERS LA English DT Article ID DIRAC SEMIMETAL CD3AS2; MAGNETIC-PROPERTIES; CADMIUM ARSENIDE; SCATTERING; GRAPHENE; SURFACE AB Cd3As2 is a candidate three-dimensional Dirac semimetal which has exceedingly high mobility and nonsaturating linear magnetoresistance that may be relevant for future practical applications. We report magnetotransport and tunnel diode oscillation measurements on Cd3As2, in magnetic fields up to 65 T and temperatures between 1.5 and 300 K. We find that the nonsaturating linear magnetoresistance persists up to 65 T and it is likely caused by disorder effects, as it scales with the high mobility rather than directly linked to Fermi surface changes even when approaching the quantum limit. From the observed quantum oscillations, we determine the bulk three-dimensional Fermi surface having signatures of Dirac behavior with a nontrivial Berry phase shift, very light effective quasiparticle masses, and clear deviations from the band-structure predictions. In very high fields we also detect signatures of large Zeeman spin splitting (g similar to 16). C1 [Narayanan, A.; Watson, M. D.; Blake, S. F.; Chen, Y. L.; Prabhakaran, D.; Coldea, A. I.] Univ Oxford, Dept Phys, Clarendon Lab, Oxford OX1 3PU, England. [Bruyant, N.; Drigo, L.; Felser, C.] CNRS, Lab Natl Champs Magnet Intenses, F-31077 Toulouse, France. [Yan, B.] Max Planck Inst Chem Phys Fester Stoffe, D-01187 Dresden, Germany. [Kong, T.; Canfield, P. C.] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. [Kong, T.; Canfield, P. C.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. RP Coldea, AI (reprint author), Univ Oxford, Dept Phys, Clarendon Lab, Parks Rd, Oxford OX1 3PU, England. EM amalia.coldea@physics.ox.ac.uk RI Narayanan, Arjun/L-7513-2015; Coldea, Amalia/C-1106-2013; Felser, Claudia/A-5779-2009; OI Narayanan, Arjun/0000-0001-6869-6997; Felser, Claudia/0000-0002-8200-2063; , /0000-0002-2269-3253; Kong, Tai/0000-0002-5064-3464; Watson, Matthew/0000-0002-0737-2814 FU EPSRC [EP/L001772/1, EP/I004475/1, EP/I017836/1]; EPSRC Career Acceleration Fellowship [EP/I004475/1]; U.S. Department of Energy, Office of Basic Energy Science, Division of Materials Sciences and Engineering; U.S. Department of Energy by Iowa State University [DE-AC02-07CH11358]; EPSRC (United Kingdom) [EP/K04074X/1]; DARPA (United States) MESO project [N66001-11-1-4105] FX We acknowledge and thank Igor Mazin for the band-structure calculations and comments on the manuscript. We acknowledge fruitful discussions with John Chalker, Steve Simon, Zohar Ringel, and Gabor Halasz and useful comments given by David Macdougal and S. L. Bud'ko. This work was mainly supported by EPSRC (EP/L001772/1, EP/I004475/1, EP/I017836/1). Part of the work was performed at the LNCMI, member of the European Magnetic Field Laboratory (EMFL). A. I. C. acknowledges an EPSRC Career Acceleration Fellowship (EP/I004475/1). Work done at Ames Lab was supported by the U.S. Department of Energy, Office of Basic Energy Science, Division of Materials Sciences and Engineering. Ames Laboratory is operated for the U.S. Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. Y.C. acknowledges the support from the EPSRC (United Kingdom) Grant No. EP/K04074X/1 and a DARPA (United States) MESO project (No. N66001-11-1-4105). NR 37 TC 64 Z9 64 U1 16 U2 123 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 19 PY 2015 VL 114 IS 11 AR 117201 DI 10.1103/PhysRevLett.114.117201 PG 5 WC Physics, Multidisciplinary SC Physics GA CD9PP UT WOS:000351430600011 PM 25839304 ER PT J AU Stupakov, G Bane, KLF Emma, P Podobedov, B AF Stupakov, G. Bane, K. L. F. Emma, P. Podobedov, B. TI Resistive wall wakefields of short bunches at cryogenic temperatures SO PHYSICAL REVIEW SPECIAL TOPICS-ACCELERATORS AND BEAMS LA English DT Article AB We present calculations of the longitudinal wakefields at cryogenic temperatures for extremely short bunches, characteristic for modern x-ray free electron lasers. The calculations are based on the equations for the surface impedance in the regime of the anomalous skin effect in metals. This paper extends and complements an earlier analysis of B. Podobedov, Phys. Rev. ST Accel. Beams 12, 044401 (2009). into the region of very high frequencies associated with bunch lengths in the micron range. We study in detail the case of a rectangular bunch distribution for parameters of interest of LCLS-II with a superconducting undulator. C1 [Stupakov, G.; Bane, K. L. F.; Emma, P.] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Podobedov, B.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Stupakov, G (reprint author), SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. RI Stupakov, Gennady/C-4904-2008 OI Stupakov, Gennady/0000-0003-2381-398X FU Department of Energy [DE-AC02-76SF00515, DE-AC02-98CH1-886] FX This work was supported by the Department of Energy, Contracts No. DE-AC02-76SF00515 and No. DE-AC02-98CH1-886. NR 15 TC 1 Z9 1 U1 1 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-4402 J9 PHYS REV SPEC TOP-AC JI Phys. Rev. Spec. Top.-Accel. Beams PD MAR 19 PY 2015 VL 18 IS 3 AR 034402 DI 10.1103/PhysRevSTAB.18.034402 PG 6 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA CD9PT UT WOS:000351431000002 ER PT J AU Holby, EF Taylor, CD AF Holby, Edward F. Taylor, Christopher D. TI Activity of N-coordinated multi-metal-atom active site structures for Pt-free oxygen reduction reaction catalysis: Role of *OH ligands SO SCIENTIFIC REPORTS LA English DT Article ID DENSITY-FUNCTIONAL THEORY; INITIO MOLECULAR-DYNAMICS; TOTAL-ENERGY CALCULATIONS; PEM FUEL-CELLS; WAVE BASIS-SET; ELECTROCATALYSTS; FE; CO; TRANSITION; DESIGN AB We report calculated oxygen reduction reaction energy pathways on multi-metal-atom structures that have previously been shown to be thermodynamically favorable. We predict that such sites have the ability to spontaneously cleave the O-2 bond and then will proceed to over-bind reaction intermediates. In particular, the *OH bound state has lower energy than the final 2 H2O state at positive potentials. Contrary to traditional surface catalysts, this *OH binding does not poison the multi-metal-atom site but acts as a modifying ligand that will spontaneously form in aqueous environments leading to new active sites that have higher catalytic activities. These *OH bound structures have the highest calculated activity to date. C1 [Holby, Edward F.] Los Alamos Natl Lab, Mat Sci & Technol Div, Los Alamos, NM 87544 USA. [Taylor, Christopher D.] DNV GL, Strateg Res & Innovat, Dublin, OH 43017 USA. [Taylor, Christopher D.] Ohio State Univ, Dept Mat Sci & Engn, Fontana Corros Ctr, Columbus, OH 43210 USA. RP Holby, EF (reprint author), Los Alamos Natl Lab, Mat Sci & Technol Div, POB 1663, Los Alamos, NM 87544 USA. EM holby@lanl.gov OI Holby, Edward/0000-0001-8419-6298 FU Los Alamos National Laboratory; U.S. Department of Energy [DE-AC528-06NA25396] FX The authors wish to thank the Los Alamos National Laboratory for funding under the Laboratory Directed Research and Development (LDRD) program and for institutional computing resources. Los Alamos National Laboratory is operated by Los Alamos National Security LLC for the National Nuclear Security Administration of the U.S. Department of Energy under contract DE-AC528-06NA25396. NR 32 TC 10 Z9 10 U1 3 U2 46 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAR 19 PY 2015 VL 5 AR 9286 DI 10.1038/srep09286 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CD7NF UT WOS:000351276500002 PM 25788358 ER PT J AU Li, CB Cao, YJ Zhang, M Wang, JH Liu, JG Shi, HQ Geng, YH AF Li, Canbing Cao, Yijia Zhang, Mi Wang, Jianhui Liu, Jianguo Shi, Haiqing Geng, Yinghui TI Hidden Benefits of Electric Vehicles for Addressing Climate Change SO SCIENTIFIC REPORTS LA English DT Article ID HEAT-ISLAND AB There is an increasingly hot debate on whether the replacement of conventional vehicles (CVs) by electric vehicles (EVs) should be delayed or accelerated since EVs require higher cost and cause more pollution than CVs in the manufacturing process. Here we reveal two hidden benefits of EVs for addressing climate change to support the imperative acceleration of replacing CVs with EVs. As EVs emit much less heat than CVs within the same mileage, the replacement can mitigate urban heat island effect (UHIE) to reduce the energy consumption of air conditioners, benefitting local and global climates. To demonstrate these effects brought by the replacement of CVs by EVs, we take Beijing, China, as an example. EVs emit only 19.8% of the total heat emitted by CVs per mile. The replacement of CVs by EVs in 2012 could have mitigated the summer heat island intensity (HII) by about 0.946 degrees C, reduced the amount of electricity consumed daily by air conditioners in buildings by 14.44 million kilowatt-hours (kWh), and reduced daily CO2 emissions by 10,686 tonnes. C1 [Li, Canbing; Cao, Yijia; Zhang, Mi; Wang, Jianhui; Shi, Haiqing; Geng, Yinghui] Hunan Univ, Coll Elect & Informat Engn, Changsha 410082, Hunan, Peoples R China. [Li, Canbing; Liu, Jianguo] Michigan State Univ, Ctr Syst Integrat & Sustainabil, E Lansing, MI 48823 USA. [Wang, Jianhui] Argonne Natl Lab, Ctr Energy Environm & Econ Syst Anal, Argonne, IL 60439 USA. RP Li, CB (reprint author), Hunan Univ, Coll Elect & Informat Engn, Changsha 410082, Hunan, Peoples R China. EM licanbing@qq.com; yjcao@hnu.edu.cn; liuji@msu.edu RI Liu, Jianguo/G-5211-2015 OI Liu, Jianguo/0000-0001-6344-0087 FU National Natural Science Foundation of China [51107036] FX This research was funded by the National Natural Science Foundation of China under Grant 51107036. NR 30 TC 1 Z9 1 U1 4 U2 33 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAR 19 PY 2015 VL 5 AR 9213 DI 10.1038/srep09213 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CD7ME UT WOS:000351273700001 PM 25790439 ER PT J AU McDonald, TM Mason, JA Kong, XQ Bloch, ED Gygi, D Dani, A Crocella, V Giordanino, F Odoh, SO Drisdell, WS Vlaisavljevich, B Dzubak, AL Poloni, R Schnell, SK Planas, N Lee, K Pascal, T Wan, LWF Prendergast, D Neaton, JB Smit, B Kortright, JB Gagliardi, L Bordiga, S Reimer, JA Long, JR AF McDonald, Thomas M. Mason, Jarad A. Kong, Xueqian Bloch, Eric D. Gygi, David Dani, Alessandro Crocella, Valentina Giordanino, Filippo Odoh, Samuel O. Drisdell, Walter S. Vlaisavljevich, Bess Dzubak, Allison L. Poloni, Roberta Schnell, Sondre K. Planas, Nora Lee, Kyuho Pascal, Tod Wan, Liwen F. Prendergast, David Neaton, Jeffrey B. Smit, Berend Kortright, Jeffrey B. Gagliardi, Laura Bordiga, Silvia Reimer, Jeffrey A. Long, Jeffrey R. TI Cooperative insertion of CO2 in diamine-appended metal-organic frameworks SO NATURE LA English DT Article ID CARBON-DIOXIDE CAPTURE; TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; COORDINATION POLYMER; POWDER DIFFRACTION; MOLECULAR-DYNAMICS; CRYSTAL-STRUCTURE; BASIS-SET; FLUE-GAS; ADSORPTION AB The process of carbon capture and sequestration has been proposed as a method of mitigating the build-up of greenhouse gases in the atmosphere. If implemented, the cost of electricity generated by a fossil fuel-burning power plant would rise substantially, owing to the expense of removing CO2 from the effluent stream. There is therefore an urgent need for more efficient gas separation technologies, such as those potentially offered by advanced solid adsorbents. Here we show that diamine-appended metal-organic frameworks can behave as 'phase-change' adsorbents, with unusual step-shaped CO2 adsorption isotherms that shift markedly with temperature. Results from spectroscopic, diffraction and computational studies show that the origin of the sharp adsorption step is an unprecedented cooperative process in which, above a metal-dependent threshold pressure, CO2 molecules insert into metal-amine bonds, inducing a reorganization of the amines into well-ordered chains of ammonium carbamate. As a consequence, large CO2 separation capacities can be achieved with small temperature swings, and regeneration energies appreciably lower than achievable withstate-of-the-art aqueous amine solutions become feasible. The results provide a mechanistic framework for designing highly efficient adsorbents for removing CO2 from various gas mixtures, and yield insights into the conservation of Mg2+ within the ribulose-1,5-bisphosphate carboxylase/oxygenase family of enzymes. C1 [McDonald, Thomas M.; Mason, Jarad A.; Bloch, Eric D.; Gygi, David; Long, Jeffrey R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Kong, Xueqian; Vlaisavljevich, Bess; Schnell, Sondre K.; Lee, Kyuho; Smit, Berend; Reimer, Jeffrey A.] Univ Calif Berkeley, Dept Chem & Biol Engn, Berkeley, CA 94720 USA. [Kong, Xueqian] Zhejiang Univ, Dept Chem, Hangzhou 310027, Zhejiang, Peoples R China. [Dani, Alessandro; Crocella, Valentina; Giordanino, Filippo; Bordiga, Silvia] Univ Turin, NIS & INSTM Ctr Reference, Dept Chem, I-10135 Turin, Italy. [Odoh, Samuel O.; Dzubak, Allison L.; Planas, Nora; Gagliardi, Laura] Univ Minnesota, Dept Chem, Chem Theory Ctr, Minneapolis, MN 55455 USA. [Odoh, Samuel O.; Dzubak, Allison L.; Planas, Nora; Gagliardi, Laura] Univ Minnesota, Supercomp Inst, Minneapolis, MN 55455 USA. [Drisdell, Walter S.; Smit, Berend; Kortright, Jeffrey B.; Reimer, Jeffrey A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA. [Poloni, Roberta] Univ Grenoble Alpes, F-38000 Grenoble, France. [Poloni, Roberta] Sci & Ingn Mat & Proc SIMAP, F-38000 Grenoble, France. [Poloni, Roberta] CNRS, SIMAP, F-38000 Grenoble, France. [Schnell, Sondre K.] Norwegian Univ Sci & Technol, Dept Chem, N-7491 Trondheim, Norway. [Pascal, Tod; Wan, Liwen F.; Prendergast, David; Neaton, Jeffrey B.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Neaton, Jeffrey B.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Neaton, Jeffrey B.] Univ Calif Berkeley, Kavli Energy Nanosci Inst, Berkeley, CA 94720 USA. [Smit, Berend] EPFL, Inst Sci & Ingn Chim, Valais, CH-1950 Sion, Switzerland. RP Long, JR (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM jrlong@berkeley.edu RI Smit, Berend/B-7580-2009; Bordiga, Silvia/M-3875-2014; Neaton, Jeffrey/F-8578-2015; Foundry, Molecular/G-9968-2014; Crocella, Valentina/E-5203-2016; Schnell, Sondre /H-4934-2016; Vlaisavljevich, Bess/Q-9737-2016 OI Smit, Berend/0000-0003-4653-8562; Bordiga, Silvia/0000-0003-2371-4156; Neaton, Jeffrey/0000-0001-7585-6135; Crocella, Valentina/0000-0002-3606-8424; Schnell, Sondre /0000-0002-0664-6756; Vlaisavljevich, Bess/0000-0001-6065-0732 FU Advanced Research Projects Agency-Energy (ARPA-E), US Department of Energy (DOE) [DE-AR0000103, DE-AR0000402]; DOE, Office of Science, Office of Basic Energy Sciences [DE-SC0001015]; GENCI (CINES) [2014-c2015097211]; Nanoporous Materials Genome Center of the DOE, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences [DE-FG02-12ER16362]; DOE Office of Science [DE-AC02-06CH11357]; Office of Science, Office of Basic Energy Sciences of the DOE [DE-AC02-05CH11231]; National Science Foundation; Research Council of Norway [230534]; [MIUR-PRIN 2010-2011] FX We thank A. S. Bhown and A. H. Berger of EPRI, H. Krutka, C. M. Brown and. K. S. Suslick for discussions, and L. Ribaud and the 11-BM staff at the Advanced Photon Source at Argonne National Laboratory for assisting with powder X-ray diffraction experiments. The work presented here pertaining to the synthesis and gas adsorption properties of metal-organic frameworks was funded by the Advanced Research Projects Agency-Energy (ARPA-E), US Department of Energy (DOE), under award numbers DE-AR0000103 and DE-AR0000402. Funding pertaining to the characterization of materials by spectroscopy and X-ray diffraction and the computational work performed by W.S.D., B.V., R.P., S.K.S., K.L., J.B.N., B.S. and J.B.K. was provided by the Center for Gas Separations Relevant to Clean Energy Technologies, an Energy Frontier Research Center funded by the DOE, Office of Science, Office of Basic Energy Sciences under award DE-SC0001015. Experiments performed in Turin were supported by grant MIUR-PRIN 2010-2011. Work at SIMAP was performed using computer resources from GENCI (CINES grant 2014-c2015097211). The computational work performed by S.O.O., A.L.D., N.P. and L.G. was supported through the Nanoporous Materials Genome Center of the DOE, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences, under award number DE-FG02-12ER16362. This research used resources of the Advanced Photon Source, a DOE Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under contract no. DE-AC02-06CH11357. Portions of this work (use of beamline 6.3.2 at the Advanced Light Source; a user project at The Molecular Foundry, facilitated by T.P., L.F.W. and D.P., and use of its computer cluster vulcan, managed by the High Performance Computing Services Group; use of the National Energy Research Scientific Computing Center) were performed at Lawrence Berkeley National Laboratory, which is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the DOE under contract no. DE-AC02-05CH11231. For fellowship support, we further thank the National Science Foundation (J.A.M.), Gerald K. Branch and Arkema (E.D.B.) and the Research Council of Norway (grant 230534 to S.K.S.). NR 62 TC 174 Z9 175 U1 83 U2 478 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD MAR 19 PY 2015 VL 519 IS 7543 BP 303 EP + DI 10.1038/nature14327 PG 16 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CD6AY UT WOS:000351171900031 PM 25762144 ER PT J AU Feldman, DR Collins, WD Gero, PJ Torn, MS Mlawer, EJ Shippert, TR AF Feldman, D. R. Collins, W. D. Gero, P. J. Torn, M. S. Mlawer, E. J. Shippert, T. R. TI Observational determination of surface radiative forcing by CO2 from 2000 to 2010 SO NATURE LA English DT Article ID EMITTED RADIANCE INTERFEROMETER; SOUTHERN GREAT-PLAINS; WATER-VAPOR FEEDBACK; CARBON-DIOXIDE; LONGWAVE RADIATION; SPECTRA; TEMPERATURE; PERFORMANCE; HUMIDITY; PROGRAM AB The climatic impact of CO2 and other greenhouse gases is usually quantified in terms of radiative forcing', calculated as the difference between estimates of the Earth's radiation field from pre-industrial and presentday concentrations of these gases. Radiative transfer models calculate that the increase in CO2 since 1750 corresponds to a global annualmean radiative forcing at the tropopause of 1.82 +/- 0.19W m(-2) (ref. 2). However, despite widespread scientific discussion and modelling of the climate impacts of well-mixed greenhouse gases, there is little direct observational evidence of the radiative impact of increasing atmospheric CO2. Here we present observationally based evidence of clear-sky CO2 surface radiative forcing that is directly attributable to the increase, between 2000 and 2010, of 22 parts per million atmospheric CO2. The time series of this forcing at the two locations the Southern Great Plains and the North Slope of Alaska are derived from Atmospheric Emitted Radiance Interferometer spectra' together with ancillary measurements and thoroughly corroborated radiative transfer calculations'. The time series both show statistically significant trends of 0.2 W m(-2) per decade (with respective uncertainties of +/- 0.06 W m(-2) per decade and 0.07 W m(-2) per decade) and have seasonal ranges of 0.1-0.2W m(-2). This is approximately ten per cent of the trend in downwelling longwave radiation'''. These results confirm theoretical predictions of the atmospheric greenhouse effect due to anthropogenic emissions, and provide empirical evidence of how rising CO2 levels, mediated by temporal variations due to photosynthesis and respiration, are affecting the surface energy balance. C1 [Feldman, D. R.; Collins, W. D.; Torn, M. S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Collins, W. D.] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. [Gero, P. J.] Univ Wisconsin, Space Sci & Engn Ctr, Madison, WI 53706 USA. [Torn, M. S.] Univ Calif Berkeley, Energy & Resources Grp, Berkeley, CA 94720 USA. [Mlawer, E. J.] Atmospher & Environm Res Inc, Lexington, MA 02141 USA. [Shippert, T. R.] Pacific NW Natl Lab, Fundamental & Computat Sci, Richland, WA 99354 USA. RP Feldman, DR (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, 1 Cyclotron Rd,MS 74R-316C, Berkeley, CA 94720 USA. EM drfeldman@lbl.gov RI Collins, William/J-3147-2014; Torn, Margaret/D-2305-2015; Feldman, Daniel/N-8703-2013 OI Collins, William/0000-0002-4463-9848; Feldman, Daniel/0000-0003-3365-5233 FU US Department of Energy, Office of Science, Office of Biological and Environmental Research, Climate and Environmental Science Division, of the US Department of Energy as part of the Atmospheric System Research Program [DE-AC02-05CH11231]; Atmospheric Radiation Measurement (ARM) Climate Research Facility Southern Great Plains; National Energy Research Scientific Computing Center (NERSC) [DE-AC02-05CH11231] FX This material is based upon work supported by the US Department of Energy, Office of Science, Office of Biological and Environmental Research, Climate and Environmental Science Division, of the US Department of Energy under Award Number DE-AC02-05CH11231 as part of the Atmospheric System Research Program and the Atmospheric Radiation Measurement (ARM) Climate Research Facility Southern Great Plains. We used resources of the National Energy Research Scientific Computing Center (NERSC) under that same award. I. Williams, W. Riley, and S. Biraud of the Lawrence Berkeley National Laboratory, and D. Turner of the National Severe Storms Laboratory also provided feedback. The Broadband Heating Rate Profile (BBHRP) runs were performed using Pacific Northwest National Laboratory (PNNL) Institutional Computing at PNNL, with help from K. Cady-Pereira of Atmospheric Environmental Research, Inc., L. Riihimaki of PNNL, and D. Troyan of Brookhaven National Laboratory. NR 46 TC 13 Z9 14 U1 10 U2 61 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD MAR 19 PY 2015 VL 519 IS 7543 BP 339 EP + DI 10.1038/nature14240 PG 16 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CD6AY UT WOS:000351171900038 PM 25731165 ER PT J AU Linger, JG Taylor, LE Baker, JO Vander Wall, T Hobdey, SE Podkaminer, K Himmel, ME Decker, SR AF Linger, Jeffrey G. Taylor, Larry E., II Baker, John O. Vander Wall, Todd Hobdey, Sarah E. Podkaminer, Kara Himmel, Michael E. Decker, Stephen R. TI A constitutive expression system for glycosyl hydrolase family 7 cellobiohydrolases in Hypocrea jecorina SO Biotechnology for Biofuels LA English DT Article DE Hypocrea jecorina; Trichoderma reesei; Cellobiohydrolase; Cellulase expression; Fungal molecular biology; Biomass hydrolysis ID TRICHODERMA-REESEI CELLULASES; GLUCOSE-CONTAINING MEDIA; SACCHAROMYCES-CEREVISIAE; TRANSFORMATION SYSTEM; PICHIA-PASTORIS; GENE-EXPRESSION; CELLULOSE; SECRETION; CEL7A; CONVERSION AB Background: One of the primary industrial-scale cellulase producers is the ascomycete fungus, Hypocrea jecorina, which produces and secretes large quantities of diverse cellulolytic enzymes. Perhaps the single most important biomass degrading enzyme is cellobiohydrolase I (cbh1 or Cel7A) due to its enzymatic proficiency in cellulose depolymerization. However, production of Cel7A with native-like properties from heterologous expression systems has proven difficult. In this study, we develop a protein expression system in H. jecorina (Trichoderma reesei) useful for production and secretion of heterologous cellobiohydrolases from glycosyl hydrolase family 7. Building upon previous work in heterologous protein expression in filamentous fungi, we have integrated a native constitutive enolase promoter with the native cbh1 signal sequence. Results: The constitutive eno promoter driving the expression of Cel7A allows growth on glucose and results in repression of the native cellulase system, severely reducing background endo-and other cellulase activity and greatly simplifying purification of the recombinant protein. Coupling this system to Delta cbh1 strain of H. jecorina ensures that only the recombinant Cel7A protein is produced. Two distinct transformant colony morphologies were observed and correlated with high and null protein production. Production levels in 'fast' transformants are roughly equivalent to those in the native QM6a strain of H. jecorina, typically in the range of 10 to 30 mg/L when grown in continuous stirred-tank fermenters. 'Slow' transformants showed no evidence of Cel7A production. Specific activity of the purified recombinant Cel7A protein is equivalent to that of native protein when assayed on pretreated corn stover, as is the thermal stability and glycosylation level. Purified Cel7A produced from growth on glucose demonstrated remarkably consistent specific activity. Purified Cel7A from the same strain grown on lactose demonstrated significantly higher variability in activity. Conclusions: The elimination of background cellulase induction provides much more consistent measured specific activity compared to a traditional cbh1 promoter system induced with lactose. This expression system provides a powerful tool for the expression and comparison of mutant and/or phylogenetically diverse cellobiohydrolases in the industrially relevant cellulase production host H. jecorina. C1 [Taylor, Larry E., II; Baker, John O.; Vander Wall, Todd; Hobdey, Sarah E.; Podkaminer, Kara; Himmel, Michael E.; Decker, Stephen R.] Natl Renewable Energy Lab, Biosci Ctr, Golden, CO 80401 USA. [Linger, Jeffrey G.] Natl Renewable Energy Lab, Natl Bioenergy Ctr, Golden, CO 80401 USA. RP Decker, SR (reprint author), Natl Renewable Energy Lab, Biosci Ctr, 16253 Denver West Pkwy, Golden, CO 80401 USA. EM steve.decker@nrel.gov FU US Department of Energy [DE-AC36-08GO28308]; DOE Office of Energy Efficiency and Renewable Energy, Bioenergy Technologies Office FX This work was supported by the US Department of Energy under Contract No. DE-AC36-08GO28308. Funding for the work was provided by the DOE Office of Energy Efficiency and Renewable Energy, Bioenergy Technologies Office. NR 35 TC 5 Z9 5 U1 2 U2 17 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1754-6834 J9 BIOTECHNOL BIOFUELS JI Biotechnol. Biofuels PD MAR 18 PY 2015 VL 8 AR 45 DI 10.1186/s13068-015-0230-2 PG 12 WC Biotechnology & Applied Microbiology; Energy & Fuels SC Biotechnology & Applied Microbiology; Energy & Fuels GA CG4QJ UT WOS:000353271000001 PM 25904982 ER PT J AU Scherpelz, P Padavic, K Murray, A Glatz, A Aranson, IS Levin, K AF Scherpelz, Peter Padavic, Karmela Murray, Andy Glatz, Andreas Aranson, Igor S. Levin, K. TI Generic equilibration dynamics of planar defects in trapped atomic superfluids SO PHYSICAL REVIEW A LA English DT Article ID BOSE-EINSTEIN CONDENSATE; DARK SOLITONS; NONLINEAR MEDIA; PROPAGATION; INSTABILITY; CREATION; WAVES; BEAMS AB We investigate equilibration processes shortly after sudden perturbations are applied to ultracold trapped superfluids. We show the similarity of phase imprinting and localized density depletion perturbations, both of which initially are found to produce "phase walls." These planar defects are associated with a sharp gradient in the phase. Importantly they relax following a quite general sequence. Our studies, based on simulations of the complex time-dependent Ginzburg-Landau equation, address the challenge posed by these experiments: how a superfluid eventually eliminates a spatially extended planar defect. The processes involved are necessarily more complex than equilibration involving simpler line vortices. An essential mechanism for relaxation involves repeated formation and loss of vortex rings near the trap edge. C1 [Scherpelz, Peter; Padavic, Karmela; Murray, Andy; Levin, K.] Univ Chicago, James Franck Inst, Chicago, IL 60637 USA. [Scherpelz, Peter; Padavic, Karmela; Murray, Andy; Levin, K.] Univ Chicago, Dept Phys, Chicago, IL 60637 USA. [Glatz, Andreas; Aranson, Igor S.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Glatz, Andreas] Univ Illinois, Dept Phys, De Kalb, IL 60115 USA. RP Scherpelz, P (reprint author), Univ Chicago, James Franck Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. EM pscherpelz@uchicago.edu OI Scherpelz, Peter/0000-0001-8185-3387 FU NSF-MRSEC [0820054]; Scientific Discovery through Advanced Computing (SciDAC) program - U.S. Department of Energy, Office of Science, Advanced Scientific Computing Research; Basic Energy Sciences, Office of Science, Materials Sciences and Engineering Division FX We are grateful to William Irvine and Adam Rancon for insightful discussions. This work was supported by NSF-MRSEC Grant No. 0820054. Work at Argonne was supported by the Scientific Discovery through Advanced Computing (SciDAC) program funded by the U.S. Department of Energy, Office of Science, Advanced Scientific Computing Research and Basic Energy Sciences, Office of Science, Materials Sciences and Engineering Division. The numerical work was performed on NIU's GPU cluster GAEA. NR 43 TC 2 Z9 2 U1 1 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1050-2947 EI 1094-1622 J9 PHYS REV A JI Phys. Rev. A PD MAR 18 PY 2015 VL 91 IS 3 AR 033621 DI 10.1103/PhysRevA.91.033621 PG 11 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA CE9CE UT WOS:000352140300008 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schofbeck, R Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, M Bansal, S Comelis, T De Wolf, EA Janssen, X Knutsson, A Lauwers, J Luyckx, S Ochesanu, S Rougny, R Van De Klundert, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Daci, N Heracleous, N Keaveney, J Lowette, S Maes, M Olbrechts, A Python, Q Strom, D Tavemier, S Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Caillol, C Clerbaux, B De Lentdecker, G Dobur, D Favart, L Gay, APR Grebenyuk, A Leonard, A Mohammadi, A Pernie, L Randle-conde, A Reis, T Seva, T Thomas, L Vander Velde, C Vanlaer, P Wang, J Zenoni, F Adler, V Beernaert, K Benucci, L Cimmino, A Costantini, S Crucy, S Dildick, S Fagot, A Garcia, G Mccartin, J Rios, AAO Ryckbosch, D Diblen, SS Sigamani, M Strobbe, N Thyssen, F Tytgat, M Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bruno, G Castello, R Caudron, A Ceard, L Da Silveira, GG Delaere, C du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Jafari, A Jez, P Komm, M Lemaitre, V Nuttens, C Pagano, D Perrini, L Pin, A Piotrzkowski, K Popov, A Quertenmont, L Selvaggi, M Marono, MV Garcia, JMV Beliy, N Caebergs, T Daubie, E Hammad, GH Alda, WL Alves, GA Brito, L Martins, MC Martins, TD Herrera, CM Pol, ME Teles, PR Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD De Souza, SF Malbouisson, H Figueiredo, DM Mimdim, L Nogima, H Da Silva, WLP Santaolalla, J Santoro, A Sznajder, A Manganote, EJT Pereira, AV Bernardes, CA Dogra, S Tomei, TRFP Gregores, EM Mercadante, PG Novaes, SF Padula, SS Aleksandrov, A Genchev, V Hadjiiska, R Iaydjiev, P Marinov, A Piperov, S Rodozov, M Sultanov, C Vutova, M Dimitrov, A Glushkov, I Litov, L Pavlov, B Petkov, PP Bian, JG Chen, GM Chen, HS Chen, M Cheng, T Du, R Jiang, CH Plestina, R Romeo, F Tao, J Wang, Z Asawatangtrakuldee, C Ban, Y Li, Q Liu, S Mao, Y Qian, SJ Wang, D Zou, W Avila, C Cabrera, A Sierra, LFC Florez, C Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Polic, D Puljak, I Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Mekterovic, D Sudic, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Bodlak, M Finger, M Finger, M Assran, Y Elgammal, S Mahmoud, MA Radi, A Kadastik, M Murumaa, M Raidal, M Tiko, A Eerola, P Fedi, G Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Kortelainen, MJ Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E Wendland, L Talvitie, J Tuuva, T Besancon, M Couderc, F Dejardin, M Denegri, D Fabbro, B Faure, JL Favaro, C Ferri, F Ganjour, S Givemaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Malcles, J Rander, J Rosowsky, A Titov, M Baffioni, S Beaudette, F Busson, P Charlot, C Dahms, T Dalchenko, M Dobrzynski, L Filipovic, N Florent, A de Cassagnac, RG Mastrolorenzo, L Mine, P Mironov, C Naranjo, IN Nguyen, M Ochando, C Paganini, P Regnard, S Salerno, R Sauvan, JB Sirois, Y Veelken, C Yilmaz, Y Zabi, A Agram, JL Andrea, J Aubin, A Bloch, D Brom, JM Chabert, EC Collard, C Conte, E Fontaine, JC Gele D Goerlach, U Goetzmann, C Le Bilian, AC Skovpen, K Van Hove, P Gadrat, S Beauceron, S Beaupere, N Boudoul, G Bouvier, E Brochet, S Montoya, CAC Chasserat, JJ Chierici, R Contardo, D Depasse, P El Mamouni, H Fan, J Fay, J Gascon, S Gouzevitch, M Ille, B Kurca, T Lethuillier, M Mirabito, L Perries, S Alvarez, JDR Sabes, D Sgandurra, L Sordini, V Vander Donckt, M Verdier, P Viret, S 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Sarangi, T. Savin, A. Smith, W. H. Taylor, D. Vuosalo, C. Woods, N. CA CMS Collaboration TI Search for long-lived particles that decay into final states containing two electrons or two muons in proton-proton collisions at root s=8Tev SO PHYSICAL REVIEW D LA English DT Article AB A search is performed for long-lived particles that decay into final states that include a pair of electrons or a pair of muons. The experimental signature is a distinctive topology consisting of a pair of charged leptons originating from a displaced secondary vertex. Events corresponding to an integrated luminosity of 19.6 (20.5) fb(-1) in the electron (muon) channel were collected with the CMS detector at the CERN LHC in proton-proton collisions at root s TeV. No significant excess is observed above standard model expectations. Upper limits on the product of the cross section and branching fraction of such a signal are presented as a function of the long-lived particle's mean proper decay length. The limits are presented in an approximately model-independent way, allowing them to be applied to a wide class of models yielding the above topology. Over much of the investigated parameter space, the limits obtained are the most stringent to date. In the specific case of a model in which a Higgs boson in the mass range 125-1000 GeV/c(2) decays into a pair of long-lived neutral bosons in the mass range 20-350 GeV= c(2), each of which can then decay to dileptons, the upper limits obtained are typically in the range 0.2-10 fb for mean proper decay lengths of the long-lived particles in the range 0.01-100 cm. In the case of the lowest Higgs mass considered (125 GeV/c(2)), the limits are in the range 2-50 fb. These limits are sensitive to Higgs boson branching fractions as low as 10(-1). C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Bergauer, T.; Dragicevic, M.; Eroe, J.; Friedl, M.; Fruehwirth, R.; Ghete, V. 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J.; Bethani, A.; Borras, K.; Burgmeier, A.; Cakir, A.; Calligaris, L.; Campbell, A.; Choudhury, S.; Costana, F.; Pardos, C. Diez; Dolinska, C.; Dooling, S.; Dorland, T.; Eckerlin, G.; Eckstein, D.; Eichhorn, T.; Flucke, G.; Garcia, J. Garay; Geiser, A.; Gunnellini, P.; Hauk, J.; Hempel, M.; Jung, H.; Kalogeropoulos, A.; Kasemann, M.; Katsas, R.; Kieseler, J.; Kleinwort, C.; Korol, I.; Kruecker, D.; Lange, W.; Leonard, J.; Lobanov, A.; Lohmann, W.; Lutz, B.; Mankel, R.; Marfin, I.; Melzer-Pellmann, I-A; Meyer, A. B.; Mittag, G.; Mnich, J.; Mussgiller, A.; Naumann-Emme, S.; Nayak, A.; Ntomari, E.; Perrey, H.; Pitzl, D.; Placakyte, R.; Raspereza, A.; Cipriano, P. M. Ribeiro; Roland, B.; Ron, E.; Sahin, M. Oe; Salfeld-Nebgen, J.; Saxena, P.; Schoerner-Sadenius, T.; Schroeder, M.; Seitz, C.; Spannagel, S.; Trevino, A. D. R. Vargas; Walsh, R.; Wissing, C.] DESY, Hamburg, Germany. [Blobel, V.; Vignali, M. Centis; Draeger, A. R.; Erfle, J.; Garutti, E.; Goebel, K.; Goerner, M.; Haller, J.; Hoffmann, M. M.; Hoeing, R. S.; Junkes, A.; Kirschenmann, H.; Klanner, R.; Kogler, R.; Lange, J.; Lapsien, T.; Lenz, T.; Marchesini, I.; Ott, J.; Peiffer, T.; Perieanu, A.; Pietsch, N.; Poehlsen, J.; Poehlsen, T.; Rathjens, D.; Sander, C.; Schettler, H.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Seidel, M.; Sola, V.; Stadie, H.; Steinbrueck, G.; Troendle, D.; Usai, E.; Vanelderen, L.; Vanhoefer, A.] Univ Hamburg, Hamburg, Germany. [Barth, C.; Baus, C.; Berger, J.; Boeser, C.; Butz, E.; Chwalek, T.; De Boer, W.; Descroix, A.; Dierlamm, A.; Feindt, M.; Frensch, F.; Giffels, M.; Gilbert, A.; Hartmann, F.; Hauth, T.; Husemann, U.; Katkov, I.; Kommayer, A.; Kuznetsova, E.; Pardo, P. Lobelle; Mozer, M. U.; Mueller, T.; Mueller, Th.; Nuernberg, A.; Quast, G.; Rabbertz, K.; Roecker, S.; Simonis, H. J.; Stober, F. M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weiler, T.; Wolf, R.] Univ Karlsruhe, Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Giakoumopoulou, V. A.; Kyriakis, A.; Loukas, D.; Markou, A.; Markou, C.; Psallidas, A.; Topsis-Giotis, I.] NCSR Demokritos, Inst Nucl & Particle Phys, Aghia Paraskevi, Greece. [Agapitos, A.; Kesisoglou, S.; Panagiotou, A.; Saoulidou, N.; Stiliaris, E.] Univ Athens, Athens, Greece. [Aslanoglou, X.; Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Manthos, N.; Papadopoulos, I.; Paradas, E.; Strologas, J.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.] Wigner Res Ctr Phys, Budapest, Hungary. [Beni, N.; Czellar, S.; Karancsi, J.; Molnar, J.; Palinkas, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Makovec, A.; Raics, P.; Trocsanyi, Z. L.; Ujvar, B.] Univ Debrecen, H-4012 Debrecen, Hungary. [Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Beri, S. B.; Bhatnagar, V.; Gupta, R.; Bhawandeep, U.; Kalsi, A. K.; Kaur, M.; Kumar, R.; Mittal, M.; Nishu, N.; Singh, J. B.] Panjab Univ, Chandigarh 160014, India. [Kumar, Ashok; Kumar, Arun; Ahuja, S.; Bhardwaj, A.; Choudhary, B. C.; Kumar, A.; Malhotra, S.; Naimuddin, M.; Ranjan, K.; Sharma, V.] Univ Delhi, Delhi 110007, India. [Banerjee, S.; Bhattacharya, S.; Chatterjee, K.; Dutta, S.; Gomber, B.; Jain, Sa; Jain, Sh; Khurana, R.; Modak, A.; Mukherjee, S.; Roy, D.; Sarkar, S.; Sharan, M.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Dutta, D.; Kailas, S.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Bombay 400085, Maharashtra, India. [Aziz, T.; Banerjee, S.; Bhowmik, S.; Chatterjee, R. M.; Dewanjee, R. K.; Dugad, S.; Ganguly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Kole, G.; Kumar, S.; Maity, M.; Majumder, G.; Mazumdar, K.; Mohanty, G. B.; Parida, B.; Sudhakar, K.; Wickramage, N.] Tata Inst Fundamental Res, Bombay 400005, Maharashtra, India. [Baklishiansohi, H.; Behnamian, H.; Etesami, S. M.; Fahim, A.; Goldouzian, R.; Khakzad, M.; Niijafabadi, M. Mohammadi; Naseri, M.; Mehdiabadi, S. Paktinat; Hosseinabadi, F. Rezaei; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Felcini, M.; Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Abbrescia, M.; Calabria, C.; Chhibra, S. S.; Colaleo, A.; Creanza, D.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; My, S.; Nuzzo, S.; Pompili, A.; Pugliese, G.; Radogna, R.; Selvaggi, G.; Sharma, A.; Silvestris, L.; Venditti, R.; Verwilligen, P.] INFN Sez Bari, Bari, Italy. [Abbrescia, M.; Calabria, C.; Chhibra, S. S.; De Palma, M.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Montanari, A.; Navarria, F. L.; Perrotta, A.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] INFN Sez Bologna, Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Navarria, F. L.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] INFN Sez Catania, Catania, Italy. [Albergo, S.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Giordano, F.] CSENSM, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gallo, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] INFN Sez Firenze, Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Fabbri, F.; Piccolo, D.] INFN Lab Nazl Frascati, Frascati, Italy. [Ferretti, R.; Ferro, F.; Lo Vetere, M.; Robutti, E.; Tosi, S.] INFN Sez Genova, Genoa, Italy. [Ferretti, R.; Lo Vetere, M.; Tosi, S.] Univ Genoa, Genoa, Italy. [Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] INFN Sez Milano Bicocca, Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Manzoni, R. A.; Martelli, A.; Marzocchi, B.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Di Guida, S.; Fabozzi, F.; Iorio, A. O. M.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.] INFN Sez Napoli, Naples, Italy. [Iorio, A. O. M.] Univ Naples Federico II, Naples, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata Potenza, Naples, Italy. [Di Guida, S.; Meola, S.] Univ G Marconi Roma, Naples, Italy. [Azzi, P.; Bacchetta, N.; Biasotto, M.; Bisello, D.; Branca, A.; Carlin, R.; Checchia, P.; Dall'Osso, M.; Dorigo, T.; Dosselli, U.; Fanzago, F.; Galanti, M.; Gasparini, U.; Giubilato, P.; Gozzelino, A.; Lacaprara, S.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Ventura, S.; Zotto, P.; Zucchetta, A.] INFN Sez Padova, Padua, Italy. [Bisello, D.; Branca, A.; Carlin, R.; Dall'Osso, M.; Galanti, M.; Gasparini, U.; Giubilato, P.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.] Univ Padua, Padua, Italy. Univ Trento Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vitulo, P.] INFN Sez Pavia, Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Saha, A.; Santocchia, A.; Spiezia, A.] INFN Sez Perugia, Perugia, Italy. [Biasini, M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Fiori, F.; Foa, L.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Moon, C. S.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] INFN Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; Donato, S.; Fiori, F.; Foa, L.; Ligabue, F.; Vernieri, C.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; D'imperio, G.; Del Re, D.; Diemoz, M.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Soffi, L.; Tracyk, P.] INFN Sez Roma, Rome, Italy. [Barone, L.; D'imperio, G.; Del Re, D.; Longo, E.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Santanastasio, F.; Soffi, L.; Tracyk, P.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Ameodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Degano, A.; Demaria, N.; Finco, L.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Ortona, G.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] INFN Sez Torino, Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Casasso, S.; Costa, M.; Degano, A.; Finco, L.; Migliore, E.; Monaco, V.; Ortona, G.; Pacher, L.; Angioni, G. L. Pinna; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Ameodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Schizzi, A.; Umer, T.; Zanetti, A.] INFN Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Schizzi, A.; Umer, T.] Univ Trieste, Trieste, Italy. [Chang, S.; Kropivnitskaya, A.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Park, H.; Sakharov, A.; Son, D. C.] Kyungpook Natl Univ, Daegu, South Korea. [Kim, T. J.] Chonbuk Natl Univ, Jeonju 561756, South Korea. [Kim, J. Y.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, Y.; Lee, B.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Yoo, H. D.] Seoul Natl Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, I. C.; Ryu, G.; Ryu, M. S.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, D.; Kwon, E.; Lee, J.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.] Vilnius State Univ, Vilnius, Lithuania. [Komaragiri, J. R.; Ali, M. A. B. Md] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Casimiro Linares, E.; Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Hernandez-Almada, A.; Lopez-Fernandez, R.; Sanchez-Hernandez, A.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Pedraza, I.; Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Reucroft, S.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, A.; Ahmad, M.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.; Wolszczak, W.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz E Silva, C.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Lloret Iglesias, L.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Varela, I.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Kozlov, G.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Savina, M.; Shmatov, S.; Shulha, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An; Andreev, Yu] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Pozdnyakov, I.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Belyaev, A.; Boos, E.; Bunichev, V.; Dubinin, M.; Dudko, L.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Obraztsov, S.; Perfilov, M.; Petrushanko, S.; Savrin, V.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia. [Adzic, P.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia. [Alcaraz Maestre, J.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olineda, A.; Redondo, I.; Romero, L.; Soares, M. S.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Graziano, A.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Bernet, C.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; David, A.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dorney, B.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Franzoni, G.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Hansen, M.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Magini, N.; Malgeri, L.; Mannelli, M.; Marrouche, J.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Orsini, L.; Pape, L.; Perez, E.; Perrozzi, L.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Pimiae, M.; Piparo, D.; Plagge, M.; Racz, A.; Rolandi, C.; Rovere, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Sharma, A.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Steggemann, J.; Stieger, B.; Stoye, M.; Takahashi, Y.; Treille, D.; Tsirou, A.; Veres, G. I.; Wardle, N.; Woehri, H. K.; Wollny, H.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Buchmann, M. A.; Casal, B.; Chanon, N.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eller, P.; Grab, C.; Hits, D.; Hoss, J.; Lustermann, W.; Mangano, B.; Marini, A. C.; Marionneau, M.; del Arbo, P. Martinez Ruiz; Masciovecchio, M.; Meister, D.; Mohr, N.; Musella, P.; Naegeli, C.; Nessi-Tedaldi, F.; Pandolfi, F.; Pauss, F.; Peruzzi, M.; Quittnat, M.; Rebane, L.; Rossini, M.; Starodumov, A.; Takahashi, M.; Theofilatos, K.; Wallny, R.; Weber, H. A.] ETH, Inst Particle Phys, Zurich, Switzerland. [Amsler, C.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Mejias, B. Milian; Ngadiuba, J.; Pinna, D.; Robmann, P.; Ronga, F. J.; Taroni, S.; Verzetti, M.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli, Taiwan. [Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Grundler, U.; Hou, W-S; Kao, K. Y.; Liu, Y. F.; Lu, R-S; Majumder, D.; Petrakou, E.; Tzeng, Y. M.; Wilken, R.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Dept Phys, Fac Sci, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Gamsizkan, H.; Isildak, B.; Karapinar, G.; Ocalan, K.; Sekmen, S.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Albayrak, E. A.; Guelmez, E.; Kaya, M.; Kaya, O.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cankocak, K.; Vardarli, F. I.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S. S.; Poll, A.; Sakuma, T.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Womersley, W. J.; Worm, S. D.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Dauncey, P.; Davies, G.; Della Negra, M.; Dunne, P.; Ferguson, W.; Fulcher, J.; Futyan, D.; Hall, G.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A-M; Malik, S.; Mathias, B.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Tapper, A. A.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL 35487 USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Lawson, P.; Richardson, C.; Rohlf, J.; St John, J.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Berry, E.; Bhattacharya, S.; Christopher, G.; Cutts, D.; Demiragli, Z.; Dhingra, N.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.; Swanson, J.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; De La Barca Sanchez, M. Calderon; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Lander, R.; Miceli, T.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Searle, M.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Cousins, R.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Rakness, G.; Takasugi, E.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA 90095 USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Rikova, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Negrete, M. Olmedo; Shrinivas, A.; Sumowidagdo, S.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Holzner, A.; Kelley, R.; Klein, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Palmer, C.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Tadel, M.; Tu, Y.; Vartak, A.; Welke, C.; Wuerthwein, F.; Yagil, A.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bradmiller-Feld, J.; Campagnari, C.; Danielson, T.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, E.; Gouskos, L.; Incandela, J.; Justus, C.; Mccoll, N.; Richman, J.; Stuart, D.; To, W.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Pierini, M.; Spiropulu, M.; Vlimant, J. R.; Wilkinson, R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Iiyama, Y.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Krohn, M.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Skinnari, L.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY 14853 USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Aleksandrov, A.; Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Kaadze, K.; Klima, B.; Kreis, B.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mishra, K.; Mrenna, S.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Sexton-Kennedy, E.; Sharma, S.; Soha, A.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitbeck, A.; Whitmore, J.; Yang, F.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Carver, M.; Curry, D.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Field, R. D.; FiSher, M.; Furic, I. K.; Hugon, J.; Konigsberg, J.; Korytov, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Rinkevicius, A.; Shchutska, L.; Snowball, M.; Sperka, D.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL 32611 USA. [Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Kurt, P.; Moon, D. H.; O'Brien, C.; Gonzalez, I. D. Sandoval; Silkworth, C.; Turner, P.; Varelas, N.] Univ Illinois Chicago UIC, Chicago, IL 60637 USA. [Bilki, B.; Clarida, W.; Dilsiz, K.; Haytmyradov, M.; Merlo, J-P; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Rahmat, R.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yi, K.; Barnett, B. A.] Univ Iowa, Iowa City, IA 52242 USA. [Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Swartz, M.] Johns Hopkins Univ, Baltimore, MD 21218 USA. [Baringer, P.; Bean, A.; Benelli, G.; Bruner, C.; Kenny, R. P., III; Malek, M.; Murray, M.; Noonan, D.; Sanders, S.; Sekaric, J.; Stringer, R.; Wang, Q.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Skhirtladze, N.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, MI 48201 USA. [Baden, A.; Belloni, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Mignerey, A. C.; Pedro, K.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Bauer, G.; Busza, W.; Cali, I. A.; Chan, M.; Di Matteo, L.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Klute, M.; Lai, Y. S.; Lee, Y-J; Levin, A.; Luckey, P. D.; Ma, T.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Velicanu, D.; Veverka, J.; Wyslouch, B.; Yang, M.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; Gude, A.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN 55455 USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, University, MS 38677 USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Suarez, R. Gonzalez; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Meier, F.; Ratnikov, F.; Snow, G. R.; Zvada, M.] Univ Nebraska, Lincoln, NE 68588 USA. [Dolen, J.; Godshalk, A.; Iashvili, I.; Kharchilava, A.; Kumar, A.; Rappoccio, S.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgarte, D.; Chasco, M.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; Trocino, D.; Wang, R-J; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Hahn, K. A.; Kubik, A.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL 60208 USA. [Brinkerhoff, A.; Chan, K. M.; Drozdetskiy, A.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Lynch, S.; Marinelli, N.; Musienko, Y.; Pearson, T.; Planer, M.; Ruchti, R.; Smith, G.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hart, A.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Luo, W.; Puigh, D.; Rodenburg, M.; Winer, B. L.; Wolfe, H.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Driga, O.; Elmer, P.; Hardenbrook, J.; Hebda, P.; Hunt, A.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Brownson, E.; Malik, S.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR 00681 USA. [Barnes, V. E.; Benedetti, D.; Bortoletto, D.; De Mattia, M.; Gutay, L.; Hu, Z.; Jha, M. K.; Jones, M.; Jung, K.; Kress, M.; Leonardo, N.; Pegna, D. Lopes; Maroussov, V.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shi, X.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.; Stupak, J.] Purdue Univ Calumet, Hammond, IA 46323 USA. [Adair, A.; Akgun, B.; Ecklund, K. M.; Geurts, F. J. M.; Li, W.; Michlin, B.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX 77251 USA. [Betchart, B.; Bodek, A.; Covarelli, R.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Khukhunaishvili, A.; Korjenevski, S.; Petrillo, G.; Vishnevskiy, D.] Univ Rochester, Rochester, NY 14627 USA. [Ciesielski, R.; Demortier, L.; Goulianos, K.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Kaplan, S.; Lath, A.; Panwalkar, S.; Park, M.; Patel, R.; Salur, S.; Schnetzer, S.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Rose, K.; Spanier, S.; York, A.] Univ Tennessee, Knoxville, TN 37996 USA. [Bouhali, O.; Hernandez, A. Castaneda; Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Khotilovich, V.; Krutelyov, V.; Montalvo, R.; Osipenkov, I.; Pakhotin, Y.; Perloff, A.; Roe, J.; Rose, A.; Safonov, A.; Suarez, I.; Tatarinov, A.; Akchurin, N.] Texas A&M Univ, College Stn, TX 77843 USA. [Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kovitanggoon, K.; Kunori, S.; Lee, S. W.; Libeiro, T.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Johns, W.; Maguire, C.; Mao, Y.; Melo, A.; Sharma, M.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN 37235 USA. [Arenton, M. W.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Li, H.; Lin, C.; Neu, C.; Wood, J.] Univ Virginia, Charlottesville, VA 22904 USA. [Clarke, C.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sturdy, J.] Wayne State Univ, Detroit, MI 48202 USA. [Belknap, D. A.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Dodd, L.; Duric, S.; Friis, E.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Lanaro, A.; Lazaridis, C.; Levine, A.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ross, I.; Sarangi, T.; Savin, A.; Smith, W. H.; Taylor, D.; Vuosalo, C.; Woods, N.] Univ Wisconsin, Madison, WI 53706 USA. [Fruehwirth, R.; Jeitler, M.; Krammer, M.; Wulz, C-E] Vienna Univ Technol, A-1040 Vienna, Austria. [Rabady, D.; Pernie, L.; Genchev, V.; Agram, J-L; Boudoul, G.; Contardo, D.; Lingemann, J.; Hartmann, F.; Kommayer, A.; Mohanty, A. K.; Radogna, R.; Silvestris, L.; Giordano, F.; Gennai, S.; Gerosa, R.; Lucchini, M. T.; Marzocchi, B.; Di Guida, S.; Meola, S.; Paolucci, P.; Ciangottini, D.; Spiezia, A.; Donato, S.; Palla, F.; Savoy-Navarro, A.; Micheli, F.; Tracyk, P.; Casasso, S.; Finco, L.; Candelise, V.; Stickland, D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Beluffi, C.] Univ Haute Alsace Mulhouse, Inst Pluridisciplinaire Hubert Curien, Univ Strasbourg, CNRS IN2P3, Strasbourg, France. [Giammanco, A.] NICPB, Tallinn, Estonia. [Popov, A.; Zhukov, V.; Katkov, I.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Chinellato, J.; Tonelli Manganote, E. J.] Univ Estadual Campinas, Campinas, Brazil. [Plestina, R.; Bernet, C.] Ecole Polytech, Lab Leprince Ringuet, IN2P3 CNRS, Palaiseau, France. [Finger, M., Jr.; Tsamalaidze, Z.] Joint Inst Nucl Res, Dubna, Russia. [Assran, Y.] Suez Univ, Suez, Egypt. [Elgammal, S.] British Univ Egypt, Cairo, Egypt. [Mahmoud, M. A.] Fayoum Univ, Al Fayyum, Egypt. [Radi, A.] Ain Shams Univ, Cairo, Egypt. [Radi, A.] Sultan Qaboos Univ, Muscat, Oman. [Conte, E.; Fontaine, J-C] Univ Haute Alsace, Mulhouse, France. [Hempel, M.; Lohmann, W.; Marfin, I.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Horvath, D.] Inst Nucl Res ATOMK1, Debrecen, Hungary. [Vesztergombi, G.; Veres, G. I.] Eotvos Lorand Univ, Budapest, Hungary. [Karancsi, J.] Univ Debrecen, Debrecen, Hungary. [Bhowmik, S.; Maity, M.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Gurtu, A.] King Abdulaziz Univ, Jeddah 21413, Saudi Arabia. [Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka. [Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Fahim, A.] Univ Tehran, Dept Engn Sci, Tehran, Iran. [Safarzadeh, B.] Islamic Azad Univ, Sci & Res Branch, Plasma Phys Res Ctr, Tehran, Iran. [Biasotto, M.] Ist Nazl Fis Nucl, Lab Nazl Legnaro, I-35020 Legnaro, Italy. [Androsov, K.; Ciocci, M. A.; Grippo, M. T.; Squillacioti, P.; Belyaev, A.] Univ Siena, I-53100 Siena, Italy. [Moon, C. S.; Milenovic, P.] CNRS IN2P3, Paris, France. [Savoy-Navarro, A.; Bilki, B.] Purdue Univ, W Lafayette, IN 47907 USA. [Heredia-de La Cruz, I.; Mermerkaya, H.] Univ Michoacana, Morelia, Michoacan, Mexico. [Matveev, V.; Marinelli, N.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Kim, V.] St Petersburg State Polytech Univ, St Petersburg, Russia. [Dubinin, M.] CALTECH, Pasadena, CA 91125 USA. [Adzic, P.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Colafranceschi, S.] Univ Rome, Fac Ingn, Rome, Italy. [Rolandi, C.] Scuola Normale Super Pisa, Pisa, Italy. [Rolandi, C.] Sez INEN, Pisa, Italy. [Sphicas, P.] Univ Athens, Athens, Greece. [Naegeli, C.] Paul Scherrer Inst, Villigen, Switzerland. [Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Bakirci, M. N.; Ozturk, S.; Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey. [Cerci, S.; Cerci, D. Sunar; Tali, B.] Adiyaman Univ, Adiyarnan, Turkey. [Onengut, G.] Cag Univ, Mersin, Turkey. [Gamsizkan, H.] Anadolu Univ, Eskisehir, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Ocalan, K.] Necmettin Erbakan Univ, Konya, Turkey. [Albayrak, E. A.; Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Kaya, M.] Marmara Univ, Istanbul, Turkey. [Kaya, O.] Kafkas Univ, Kars, Turkey. [Yetkin, T.] Yildiz Tekn Univ, Istanbul, Turkey. [Newbold, D. M.; Lucas, R.] Rutherford Appleton Lab, Dideot, England. [Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. Vinca Inst Nucl Sci, Belgrade, Serbia. Argonne Natl Lab, Argonne, IL 60439 USA. Erzincan Univ, Erzincan, Turkey. [Bouhali, O.] Texas A&M Univ Qatar, Doha, Qatar. [Kamon, T.] Kyungpook Natl Univ, Daegu, South Korea. RP Khachatryan, V (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Manganote, Edmilson/K-8251-2013; candelise, vieri/H-2195-2015; Montanari, Alessandro/J-2420-2012; VARDARLI, Fuat Ilkehan/B-6360-2013; Lokhtin, Igor/D-7004-2012; Sen, Sercan/C-6473-2014; D'Alessandro, Raffaello/F-5897-2015; Petrushanko, Sergey/D-6880-2012; Wulz, Claudia-Elisabeth/H-5657-2011; Belyaev, Alexander/F-6637-2015; Stahl, Achim/E-8846-2011; Trocsanyi, Zoltan/A-5598-2009; Cavallo, Nicola/F-8913-2012; Rolandi, Luigi (Gigi)/E-8563-2013; Sguazzoni, Giacomo/J-4620-2015; Ligabue, Franco/F-3432-2014; Hernandez Calama, Jose Maria/H-9127-2015; Grandi, Claudio/B-5654-2015; Ragazzi, Stefano/D-2463-2009; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Flix, Josep/G-5414-2012; Andreev, Vladimir/M-8665-2015; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Ogul, Hasan/S-7951-2016; Dremin, Igor/K-8053-2015; Paulini, Manfred/N-7794-2014; Della Ricca, Giuseppe/B-6826-2013; Tinoco Mendes, Andre David/D-4314-2011; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Da Silveira, Gustavo Gil/N-7279-2014; Mora Herrera, Maria Clemencia/L-3893-2016; Mundim, Luiz/A-1291-2012; TUVE', Cristina/P-3933-2015; Haj Ahmad, Wael/E-6738-2016; Konecki, Marcin/G-4164-2015; ciocci, maria agnese /I-2153-2015; Marco, Jesus/B-8735-2008; My, Salvatore/I-5160-2015; Lo Vetere, Maurizio/J-5049-2012; Dogra, Sunil /B-5330-2013; Matorras, Francisco/I-4983-2015; Gennai, Simone/P-2880-2015; KIM, Tae Jeong/P-7848-2015; Menasce, Dario/A-2168-2016; Azarkin, Maxim/N-2578-2015; Cerrada, Marcos/J-6934-2014; Perez-Calero Yzquierdo, Antonio/F-2235-2013 OI Montanari, Alessandro/0000-0003-2748-6373; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Belyaev, Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279; Fiorendi, Sara/0000-0003-3273-9419; Martelli, Arabella/0000-0003-3530-2255; Gonzi, Sandro/0000-0003-4754-645X; Levchenko, Petr/0000-0003-4913-0538; Heath, Helen/0000-0001-6576-9740; Giubilato, Piero/0000-0003-4358-5355; Gallinaro, Michele/0000-0003-1261-2277; Tabarelli de Fatis, Tommaso/0000-0001-6262-4685; Rolandi, Luigi (Gigi)/0000-0002-0635-274X; Sguazzoni, Giacomo/0000-0002-0791-3350; Casarsa, Massimo/0000-0002-1353-8964; Ligabue, Franco/0000-0002-1549-7107; Diemoz, Marcella/0000-0002-3810-8530; Tricomi, Alessia Rita/0000-0002-5071-5501; Martinez Ruiz del Arbol, Pablo/0000-0002-7737-5121; Ghezzi, Alessio/0000-0002-8184-7953; Demaria, Natale/0000-0003-0743-9465; Benaglia, Andrea Davide/0000-0003-1124-8450; Covarelli, Roberto/0000-0003-1216-5235; Ciulli, Vitaliano/0000-0003-1947-3396; Androsov, Konstantin/0000-0003-2694-6542; Hernandez Calama, Jose Maria/0000-0001-6436-7547; Grandi, Claudio/0000-0001-5998-3070; Longo, Egidio/0000-0001-6238-6787; Di Matteo, Leonardo/0000-0001-6698-1735; Baarmand, Marc/0000-0002-9792-8619; Boccali, Tommaso/0000-0002-9930-9299; Ragazzi, Stefano/0000-0001-8219-2074; Gerosa, Raffaele/0000-0001-8359-3734; Attia Mahmoud, Mohammed/0000-0001-8692-5458; Bilki, Burak/0000-0001-9515-3306; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Flix, Josep/0000-0003-2688-8047; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Ogul, Hasan/0000-0002-5121-2893; Paulini, Manfred/0000-0002-6714-5787; Hu, Zhen/0000-0001-8209-4343; Della Ricca, Giuseppe/0000-0003-2831-6982; Tinoco Mendes, Andre David/0000-0001-5854-7699; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Mundim, Luiz/0000-0001-9964-7805; TUVE', Cristina/0000-0003-0739-3153; Haj Ahmad, Wael/0000-0003-1491-0446; Konecki, Marcin/0000-0001-9482-4841; ciocci, maria agnese /0000-0003-0002-5462; Marco, Jesus/0000-0001-7914-8494; My, Salvatore/0000-0002-9938-2680; Lo Vetere, Maurizio/0000-0002-6520-4480; Matorras, Francisco/0000-0003-4295-5668; KIM, Tae Jeong/0000-0001-8336-2434; Menasce, Dario/0000-0002-9918-1686; Cerrada, Marcos/0000-0003-0112-1691; Perez-Calero Yzquierdo, Antonio/0000-0003-3036-7965 FU BMWFW (Austria); FWF (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MES (Bulgaria); CERN; CAS (China); MoST (China); NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); CSF (Croatia); RPF (Cyprus); MoER (Estonia); ERC IUT (Estonia); ERDF (Estonia); Academy of Finland (Finland); MEC (Finland); HIP (Finland); CEA (France); CNRS/IN2P3 (France); BMBF (Germany); DFG (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NIH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); MSIP (Republic of Korea); NRF (Republic of Korea); LAS (Lithuania); MOE (Malaysia); UM (Malaysia); CINVESTAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE (Poland); NSC (Poland); FCT (Portugal); JINR (Dubna); MON (Russia); RosAtom (Russia); RAS (Russia); RFBR (Russia); MESTD (Serbia); SEIDI (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter (Thailand); IPST (Thailand); STAR (Thailand); NSTDA (Thailand); TUBITAK (Turkey); TAEK (Turkey); NASU (Ukraine); SFFR (Ukraine); STFC (United Kingdom); DOE (USA); NSF (USA); Marie Curie program (European Union); European Research Council (European Union); EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS program of Foundation for Polish Science; European Union, Regional Development Fund; Compagnia di San Paolo (Torino); Consorzio per la Fisica (Trieste); MIUR (Italy) [20108T4XTM]; Thalis programme; Aristeia programme; EU-ESF; Greek NSRF; National Priorities Research Program by Qatar National Research Fund FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWFW and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES and CSF (Croatia); RPF (Cyprus); MoER, ERC IUT and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NIH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); MSIP and NRF (Republic of Korea); LAS (Lithuania); MOE and UM (Malaysia); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Dubna); MON, RosAtom, RAS and RFBR (Russia); MESTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter, IPST, STAR and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU and SFFR (Ukraine); STFC (United Kingdom); DOE and NSF (USA). Individuals have received support from the Marie Curie program and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS program of Foundation for Polish Science, cofinanced by the European Union, Regional Development Fund; the Compagnia di San Paolo (Torino); the Consorzio per la Fisica (Trieste); MIUR Grant No. 20108T4XTM (Italy); the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF; and the National Priorities Research Program by Qatar National Research Fund. NR 31 TC 10 Z9 10 U1 18 U2 85 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD MAR 18 PY 2015 VL 91 IS 5 AR 052012 DI 10.1103/PhysRevD.91.052012 PG 26 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CE9HI UT WOS:000352154400001 ER PT J AU Agnese, R Anderson, AJ Balakishiyeva, D Thakur, RB Bauer, DA Billard, J Borgland, A Bowles, MA Brandt, D Brink, PL Bunker, R Cabrera, B Caldwell, DO Cerdeno, DG Chagani, H Chen, Y Cooley, J Cornell, B Crewdson, CH Cushman, P Daal, M Di Stefano, PCF Doughty, T Esteban, L Fallows, S Figueroa-Feliciano, E Godfrey, GL Golwala, SR Hall, J Harris, HR Hertel, SA Hofer, T Holmgren, D Hsu, L Huber, ME Jastram, A Kamaev, O Kara, B Kelsey, MH Kennedy, A Kiveni, M Koch, K Leder, A Loer, B Asamar, EL Mahapatra, R Mandic, V Martinez, C McCarthy, KA Mirabolfathi, N Moffatt, RA Moore, DC Nelson, H Nelson, RH Ogburn, RW Page, K Page, A Partridge, R Pepin, M Phipps, A Prasad, K Pyle, M Qiu, H Rau, W Redl, P Reisetter, A Ricci, Y Rogers, HE Saab, T Sadoulet, B Sander, J Schneck, K Schnee, RW Scorza, S Serfass, B Shank, B Speller, D Upadhyayula, S Villano, AN Welliver, B Wright, DH Yellin, S Yen, JJ Young, BA Zhang, J AF Agnese, R. Anderson, A. J. Balakishiyeva, D. Thakur, R. Basu Bauer, D. A. Billard, J. Borgland, A. Bowles, M. A. Brandt, D. Brink, P. L. Bunker, R. Cabrera, B. Caldwell, D. O. Cerdeno, D. G. Chagani, H. Chen, Y. Cooley, J. Cornell, B. Crewdson, C. H. Cushman, P. Daal, M. Di Stefano, P. C. F. Doughty, T. Esteban, L. Fallows, S. Figueroa-Feliciano, E. Godfrey, G. L. Golwala, S. R. Hall, J. Harris, H. R. Hertel, S. A. Hofer, T. Holmgren, D. Hsu, L. Huber, M. E. Jastram, A. Kamaev, O. Kara, B. Kelsey, M. H. Kennedy, A. Kiveni, M. Koch, K. Leder, A. Loer, B. Lopez Asamar, E. Mahapatra, R. Mandic, V. Martinez, C. McCarthy, K. A. Mirabolfathi, N. Moffatt, R. A. Moore, D. C. Nelson, H. Nelson, R. H. Ogburn, R. W. Page, K. Page, A. Partridge, R. Pepin, M. Phipps, A. Prasad, K. Pyle, M. Qiu, H. Rau, W. Redl, P. Reisetter, A. Ricci, Y. Rogers, H. E. Saab, T. Sadoulet, B. Sander, J. Schneck, K. Schnee, R. W. Scorza, S. Serfass, B. Shank, B. Speller, D. Upadhyayula, S. Villano, A. N. Welliver, B. Wright, D. H. Yellin, S. Yen, J. J. Young, B. A. Zhang, J. CA CDMS Collaboration TI First Direct Limits on Lightly Ionizing Particles with Electric Charge Less than e/6 SO PHYSICAL REVIEW LETTERS LA English DT Article ID SEARCH AB While the standard model of particle physics does not include free particles with fractional charge, experimental searches have not ruled out their existence. We report results from the Cryogenic Dark Matter Search (CDMS II) experiment that give the first direct-detection limits for cosmogenically produced relativistic particles with electric charge lower than e/6. A search for tracks in the six stacked detectors of each of two of the CDMS II towers finds no candidates, thereby excluding new parameter space for particles with electric charges between e/6 and e/200. C1 [Agnese, R.; Balakishiyeva, D.; Saab, T.; Welliver, B.] Univ Florida, Dept Phys, Gainesville, FL 32611 USA. [Anderson, A. J.; Billard, J.; Figueroa-Feliciano, E.; Hertel, S. A.; Leder, A.; McCarthy, K. A.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Thakur, R. Basu; Bauer, D. A.; Holmgren, D.; Hsu, L.; Loer, B.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Thakur, R. Basu] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Borgland, A.; Brandt, D.; Brink, P. L.; Godfrey, G. L.; Kelsey, M. H.; Ogburn, R. W.; Partridge, R.; Schneck, K.; Wright, D. H.] SLAC Natl Accelerator Lab, Kavli Inst Particle Astrophys & Cosmol, Menlo Pk, CA 94025 USA. [Bowles, M. A.; Bunker, R.; Chen, Y.; Kiveni, M.; Schnee, R. W.] Syracuse Univ, Dept Phys, Syracuse, NY 13244 USA. [Cabrera, B.; Moffatt, R. A.; Redl, P.; Shank, B.; Yellin, S.; Yen, J. J.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Caldwell, D. O.; Nelson, H.] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA. [Cerdeno, D. G.; Esteban, L.; Lopez Asamar, E.] Univ Autonoma Madrid, Dept Fis Teor, E-28049 Madrid, Spain. [Cerdeno, D. G.; Esteban, L.; Lopez Asamar, E.] Univ Autonoma Madrid, CSIC, Inst Fis Teor, E-28049 Madrid, Spain. [Chagani, H.; Cushman, P.; Fallows, S.; Hofer, T.; Kennedy, A.; Koch, K.; Mandic, V.; Pepin, M.; Rogers, H. E.; Villano, A. N.; Zhang, J.] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Cooley, J.; Kara, B.; Qiu, H.; Scorza, S.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Cornell, B.; Golwala, S. R.; Moore, D. C.; Nelson, R. H.] CALTECH, Div Phys Math & Astron, Pasadena, CA 91125 USA. [Crewdson, C. H.; Di Stefano, P. C. F.; Kamaev, O.; Martinez, C.; Page, K.; Rau, W.; Ricci, Y.] Queens Univ, Dept Phys, Kingston, ON K7L 3N6, Canada. [Daal, M.; Doughty, T.; Mirabolfathi, N.; Phipps, A.; Pyle, M.; Sadoulet, B.; Serfass, B.; Speller, D.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Hall, J.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Harris, H. R.; Jastram, A.; Mahapatra, R.; Prasad, K.; Sander, J.; Upadhyayula, S.] Texas A&M Univ, Dept Phys & Astron, College Stn, TX 77843 USA. [Huber, M. E.] Univ Colorado, Dept Phys, Denver, CO 80217 USA. [Page, A.] Univ British Columbia, Dept Phys & Astron, Vancouver, BC V6T 1Z1, Canada. [Reisetter, A.] Univ Evansville, Dept Phys, Evansville, IN 47722 USA. [Sadoulet, B.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Sander, J.] Univ S Dakota, Dept Phys, Vermillion, SD 57069 USA. [Young, B. A.] Santa Clara Univ, Dept Phys, Santa Clara, CA 95053 USA. [Bunker, R.; Schnee, R. W.] South Dakota Sch Mines & Technol, Dept Phys, Rapid City, SD 57701 USA. [Cerdeno, D. G.] Univ Durham, Dept Phys, IPPP, Durham DH1 3LE, England. [Scorza, S.] Karlsruhe Inst Technol, Inst Expt Kernphys, D-76128 Karlsruhe, Germany. RP Agnese, R (reprint author), Univ Florida, Dept Phys, Gainesville, FL 32611 USA. RI Hall, Jeter/E-9294-2015; Pyle, Matt/E-7348-2015; OI Pyle, Matt/0000-0002-3490-6754; Cerdeno, David G./0000-0002-7649-1956 FU National Science Foundation; U.S. Department of Energy; NSERC Canada; MultiDark (Spanish MINECO); Fermi Research Alliance, LLC [De-AC02-07CH11359]; U.S. Department of Energy [DE-AC02-76SF00515] FX The CDMS Collaboration gratefully acknowledges the contributions of numerous engineers and technicians; we would like to especially thank Dennis Seitz, Jim Beaty, Bruce Hines, Larry Novak, Richard Schmitt, Astrid Tomada, and John Emes. In addition, we gratefully acknowledge assistance from the staff of the Soudan Underground Laboratory and the Minnesota Department of Natural Resources. This work is supported in part by the National Science Foundation, by the U.S. Department of Energy, by NSERC Canada, and by MultiDark (Spanish MINECO). Fermilab is operated by the Fermi Research Alliance, LLC under Contract No. De-AC02-07CH11359. SLAC is operated under Contract No. DE-AC02-76SF00515 with the U.S. Department of Energy. NR 18 TC 1 Z9 1 U1 4 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 18 PY 2015 VL 114 IS 11 AR 111302 DI 10.1103/PhysRevLett.114.111302 PG 5 WC Physics, Multidisciplinary SC Physics GA CE9VW UT WOS:000352192500004 PM 25839256 ER PT J AU Marino, R Pouquet, A Rosenberg, D AF Marino, R. Pouquet, A. Rosenberg, D. TI Resolving the Paradox of Oceanic Large-Scale Balance and Small-Scale Mixing SO PHYSICAL REVIEW LETTERS LA English DT Article ID ROTATING STRATIFIED TURBULENCE; 2-DIMENSIONAL TURBULENCE; ENERGY-DISSIPATION; INVERSE CASCADES; INTERNAL WAVES; SOUTHERN-OCEAN; SOLAR-WIND; FLOWS; TRANSITION; RESOLUTION AB A puzzle of oceanic dynamics is the contrast between the observed geostrophic balance, involving gravity, pressure gradient, and Coriolis forces, and the necessary turbulent transport: in the former case, energy flows to large scales, leading to spectral condensation, whereas in the latter, it is transferred to small scales, where dissipation prevails. The known bidirectional constant-flux energy cascade maintaining both geostrophic balance and mixing tends towards flux equilibration as turbulence strengthens, contradicting models and recent observations which find a dominant large-scale flux. Analyzing a large ensemble of high-resolution direct numerical simulations of the Boussinesq equations in the presence of rotation and no salinity, we show that the ratio of the dual energy flux to large and to small scales agrees with observations, and we predict that it scales with the inverse of the Froude and Rossby numbers when stratification is (realistically) stronger than rotation. Furthermore, we show that the kinetic and potential energies separately undergo a bidirectional transfer to larger and smaller scales. Altogether, this allows for small-scale mixing which drives the global oceanic circulation and will thus potentially lead to more accurate modeling of climate dynamics. C1 [Marino, R.; Pouquet, A.] Natl Ctr Atmospher Res, Boulder, CO 80307 USA. [Marino, R.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Marino, R.] CNR, Inst Chem Phys Proc IPCF, I-87036 Arcavacata Di Rende, CS, Italy. [Pouquet, A.] Univ Colorado, Lab Atmospher & Space Phys, Boulder, CO 80309 USA. [Rosenberg, D.] Oak Ridge Natl Lab, Natl Ctr Computat Sci, Oak Ridge, TN 37831 USA. RP Marino, R (reprint author), Natl Ctr Atmospher Res, POB 3000, Boulder, CO 80307 USA. RI Marino, Raffaele/M-5130-2015 OI Marino, Raffaele/0000-0002-7372-8620 FU Regional Operative Program Calabria ESF; Marie Curie Project [FP7PIRSES-2010-269297-Turbo-plasmas]; DOE Office of Science [DE-AC05-00OR22725]; NSF; [NSF/CMG/1025183] FX This work was supported by NSF/CMG/1025183, Regional Operative Program Calabria ESF 2007/2013, and Marie Curie Project FP7PIRSES-2010-269297-Turbo-plasmas. It used resources of the ORNL/OLCF, which is supported by the DOE Office of Science under Contract No. DE-AC05-00OR22725. Computer time was provided by ASD at NCAR, which is supported by NSF. NR 39 TC 10 Z9 10 U1 4 U2 16 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 18 PY 2015 VL 114 IS 11 AR 114504 DI 10.1103/PhysRevLett.114.114504 PG 5 WC Physics, Multidisciplinary SC Physics GA CE9VW UT WOS:000352192500009 PM 25839278 ER PT J AU Huang, JH Cheng, L Assary, RS Wang, PQ Xue, Z Burrell, AK Curtiss, LA Zhang, L AF Huang, Jinhua Cheng, Lei Assary, Rajeev S. Wang, Peiqi Xue, Zheng Burrell, Anthony K. Curtiss, Larry A. Zhang, Lu TI Liquid Catholyte Molecules for Nonaqueous Redox Flow Batteries SO ADVANCED ENERGY MATERIALS LA English DT Article DE catholytes; electrochemistry; nonaqueous redox flow batteries; redox-active molecules; rational molecular design ID LITHIUM-ION BATTERIES; RESEARCH-AND-DEVELOPMENT; OVERCHARGE PROTECTION; ENERGY-STORAGE; ELECTROLYTES; SHUTTLE; CELL; DIFFUSION; PROGRESS C1 [Huang, Jinhua; Wang, Peiqi; Xue, Zheng; Burrell, Anthony K.; Zhang, Lu] Chem Sci & Engn Div, Argonne, IL 60439 USA. [Cheng, Lei; Assary, Rajeev S.; Curtiss, Larry A.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Zhang, L (reprint author), Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM luzhang@anl.gov RI Surendran Assary, Rajeev/E-6833-2012 OI Surendran Assary, Rajeev/0000-0002-9571-3307 FU Joint Center for Energy Storage Research (JCESR), an Energy Innovation Hub - U.S. Department of Energy, Office of Science, Basic Energy Sciences FX This work was supported as part of the Joint Center for Energy Storage Research (JCESR), an Energy Innovation Hub funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences. NR 30 TC 22 Z9 22 U1 7 U2 79 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1614-6832 EI 1614-6840 J9 ADV ENERGY MATER JI Adv. Energy Mater. PD MAR 18 PY 2015 VL 5 IS 6 AR 1401782 DI 10.1002/aenm.201401782 PG 6 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Energy & Fuels; Materials Science; Physics GA CE1ZZ UT WOS:000351613200015 ER PT J AU Li, JC Dudney, NJ Xiao, XC Cheng, YT Liang, CD Verbrugge, MW AF Li, Juchuan Dudney, Nancy J. Xiao, Xingcheng Cheng, Yang-Tse Liang, Chengdu Verbrugge, Mark W. TI Asymmetric Rate Behavior of Si Anodes for Lithium-Ion Batteries: Ultrafast De-Lithiation versus Sluggish Lithiation at High Current Densities SO ADVANCED ENERGY MATERIALS LA English DT Article DE lithium-ion batteries; silicon; electrodes; rate performance; kinetics; diffusion ID DIFFUSION-INDUCED STRESS; THIN-FILM ELECTRODES; NEGATIVE ELECTRODES; AMORPHOUS-SILICON; PERFORMANCE; INSERTION; ELECTROLYTES; DEPENDENCE; PARTICLES; EVOLUTION AB The combined effect of lithium-ion diffusion, potential-concentration gradient, and stress plays a critical role in the rate capability and cycle life of Si-based anodes of lithium-ion batteries. In this work, Si nanofilm anodes are shown to exhibit an asymmetric rate performance: around 72% of the total available capacity can be delivered during de-lithiation under a high current density of 420 A g(-1) (100C where C is the charge-rate) in 22 s; in striking contrast, only 1% capacity can be delivered during lithiation. A mathematical model of single-ion diffusion is established to elucidate the asymmetric rate performance, which can be mainly attributed to the potential-concentration profile associated with the active material and the ohmic voltage shift under high currents; the difference in chemical diffusion coefficients during lithiation and de-lithiation also plays a role. This clarifies that the charge and discharge rates of lithium-ion-battery electrodes should be evaluated separately due to the asymmetric effect in the electrochemical system. C1 [Li, Juchuan; Dudney, Nancy J.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Xiao, Xingcheng; Verbrugge, Mark W.] Gen Motors Res & Dev Ctr, Chem & Mat Syst Lab, Warren, MI 48090 USA. [Cheng, Yang-Tse] Univ Kentucky, Dept Chem & Mat Engn, Lexington, KY 40506 USA. [Liang, Chengdu] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Dudney, NJ (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. EM dudneynj@ornl.gov; Xingcheng.xiao@gm.com RI Li, Juchuan/A-2992-2009; Dudney, Nancy/I-6361-2016; Cheng, Yang-Tse/B-5424-2012 OI Li, Juchuan/0000-0002-6587-5591; Dudney, Nancy/0000-0001-7729-6178; FU Vehicle Technologies Office of the U.S. Department of Energy under the Batteries for Advanced Transportation Technologies (BATT) Program [DE-AC02-05CH11231, 7056410] FX The modeling of ionic conductivity and electrode kinetics was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. X.X. and Y.-T.C. acknowledge the support of the Assistant Secretary for Energy Efficiency and Renewable Energy, Vehicle Technologies Office of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231, subcontract No. 7056410 under the Batteries for Advanced Transportation Technologies (BATT) Program. NR 51 TC 14 Z9 14 U1 11 U2 105 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1614-6832 EI 1614-6840 J9 ADV ENERGY MATER JI Adv. Energy Mater. PD MAR 18 PY 2015 VL 5 IS 6 AR 1401627 DI 10.1002/aenm.201401627 PG 6 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Energy & Fuels; Materials Science; Physics GA CE1ZZ UT WOS:000351613200007 ER PT J AU Bloch, ED Queen, WL Chavan, S Wheatley, PS Zadrozny, JM Morris, R Brown, CM Lamberti, C Bordiga, S Long, JR AF Bloch, Eric D. Queen, Wendy L. Chavan, Sachin Wheatley, Paul S. Zadrozny, Joseph M. Morris, Russell Brown, Craig M. Lamberti, Carlo Bordiga, Silvia Long, Jeffrey R. TI Gradual Release of Strongly Bound Nitric Oxide from Fe-2(NO)(2)(dobdc) SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID METAL-ORGANIC FRAMEWORKS; SMALL MOLECULES; CARBON-DIOXIDE; HIGH-CAPACITY; ADSORPTION; CATALYSTS; STORAGE; COORDINATION; TEMPERATURE; REACTIVITY AB An iron(II)-based metal-organic framework featuring coordinatively unsaturated redox-active metal cation sites, Fe-2(dobdc) (dobdc(4-) = 2,5-dioxido-1,4-benzenedicarboxylate), is shown to strongly bind nitric oxide at 298 K. Adsorption isotherms indicate an adsorption capacity greater than 16 wt %, corresponding to the adsorption of one NO molecule per iron center. Infrared, UV-vis, and Mossbauer spectroscopies, together with magnetic susceptibility data, confirm the strong binding is a result of electron transfer from the Fe-II sites to form Fe-III-NO- adducts. Consistent with these results, powder neutron diffraction experiments indicate that NO is bound to the iron centers of the framework with an Fe-N-O separation of 1.77(1) angstrom and an FeNO angle of 150.9(5)degrees. The nitric oxide-containing material, Fe-2(NO)(2)(dobdc), steadily releases bound NO under humid conditions over the course of more than 10 days, suggesting it, and potential future iron(II)-based metal-organic frameworks, are good candidates for certain biomedical applications. C1 [Bloch, Eric D.; Zadrozny, Joseph M.; Long, Jeffrey R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Queen, Wendy L.; Brown, Craig M.] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Queen, Wendy L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Chavan, Sachin; Lamberti, Carlo; Bordiga, Silvia] Univ Turin, Dept Chem, NIS, CrisDi, I-10135 Turin, Italy. [Chavan, Sachin; Lamberti, Carlo; Bordiga, Silvia] Univ Turin, INSTM Ctr Reference, I-10135 Turin, Italy. [Wheatley, Paul S.; Morris, Russell] Univ St Andrews, EaStChem Sch Chem, St Andrews KY16 9ST, Fife, Scotland. [Brown, Craig M.] Univ Delaware, Dept Chem Engn, Newark, DE 19716 USA. [Brown, Craig M.] Australian Nucl Sci & Technol Org, Bragg Inst, Menai, NSW 2234, Australia. [Lamberti, Carlo] Southern Fed Univ, Rostov Na Donu 344090, Russia. RP Long, JR (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM jrlong@berkeley.edu RI Zadrozny, Joseph/D-8206-2015; Brown, Craig/B-5430-2009; Morris, Russell/G-4285-2010; Lamberti, Carlo/C-5901-2013; Bordiga, Silvia/M-3875-2014; Foundry, Molecular/G-9968-2014; Chavan, Sachin/B-8025-2014; Zadrozny, Joseph/A-1429-2017 OI Zadrozny, Joseph/0000-0002-1309-6545; Brown, Craig/0000-0002-9637-9355; Morris, Russell/0000-0001-7809-0315; Queen, Wendy/0000-0002-8375-2341; Lamberti, Carlo/0000-0001-8004-2312; Bordiga, Silvia/0000-0003-2371-4156; Zadrozny, Joseph/0000-0002-1309-6545 FU Center for Gas Separations Relevant to Clean Energy Technologies, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001015]; Arkema and Gerald K. Branch; Ateneo Project [ORTO11RRT5]; Mega-grant of the Russian Federation Government [14.Y26.31.0001] FX This research was supported through the Center for Gas Separations Relevant to Clean Energy Technologies, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under award DE-SC0001015. We thank Arkema and Gerald K. Branch for fellowship support of E.D.B. and Ateneo Project 2011 ORTO11RRT5 for financial support of S.B., C.L., and S.C. C.L. acknowledges the Mega-grant of the Russian Federation Government number 14.Y26.31.0001 for support. NR 58 TC 11 Z9 12 U1 5 U2 89 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAR 18 PY 2015 VL 137 IS 10 BP 3466 EP 3469 DI 10.1021/ja5132243 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA CD9LW UT WOS:000351420800007 PM 25710124 ER PT J AU Yang, M Liu, JL Lee, S Zugic, B Huang, J Allard, LF Flytzani-Stephanopoulos, M AF Yang, Ming Liu, Jilei Lee, Sungsik Zugic, Branko Huang, Jun Allard, Lawrence F. Flytzani-Stephanopoulos, Maria TI A Common Single-Site Pt(II)-O(OH)(x)- Species Stabilized by Sodium on "Active" and "Inert" Supports Catalyzes the Water-Gas Shift Reaction SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID C-H BOND; PLATINUM CATALYSTS; PERFORMANCE; FORMATE; ATOMS; LTL AB While it has long been known that different types of support oxides have different capabilities to anchor metals and thus tailor the catalytic behavior, it is not always clear whether the support is a mere carrier of the active metal site, itself not participating directly in the reaction pathway. We report that catalytically similar single-atom-centric Pt sites are formed by binding to sodium ions through -O ligands, the ensemble being equally effective on supports as diverse as TiO2, L-zeolites, and mesoporous silica MCM-41. Loading of 0.5 wt % Pt on all of these supports preserves the Pt in atomic dispersion as Pt(II), and the Pt-O(OH)(x)- species catalyzes the water-gas shift reaction from similar to 120 to 400 degrees C. Since the effect of the support is indirect, these findings pave the way for the use of a variety of earth-abundant supports as carriers of atomically dispersed platinum for applications in catalytic fuel-gas processing. C1 [Yang, Ming; Liu, Jilei; Zugic, Branko; Flytzani-Stephanopoulos, Maria] Tufts Univ, Dept Chem & Biol Engn, Medford, MA 02155 USA. [Lee, Sungsik] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. [Huang, Jun] Univ Sydney, Sch Chem & Biomol Engn, Sydney, NSW 2006, Australia. [Allard, Lawrence F.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Flytzani-Stephanopoulos, M (reprint author), Tufts Univ, Dept Chem & Biol Engn, Medford, MA 02155 USA. EM maria.flytzani-stephanopoulos@tufts.edu RI Huang, Jun /D-6959-2013 FU Department of Energy/Basic Energy Science [DE-FG02-05ER15730]; Advanced Photon Source at Argonne National Laboratory [DE-AC02-06CH11357]; U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Vehicle Technologies Office, Propulsion Materials Program; USyd Early Career Researcher Scheme FX Financial support by Department of Energy/Basic Energy Science under Grant DE-FG02-05ER15730 is gratefully acknowledged. The XAS research was sponsored by the Advanced Photon Source at Argonne National Laboratory under Contract DE-AC02-06CH11357. Microscopy research was sponsored by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Vehicle Technologies Office, Propulsion Materials Program. Work at Sydney was supported by the USyd Early Career Researcher Scheme. NR 21 TC 38 Z9 38 U1 37 U2 134 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAR 18 PY 2015 VL 137 IS 10 BP 3470 EP 3473 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA CD9LW UT WOS:000351420800008 PM 25746682 ER PT J AU Jarry, A Gottis, S Yu, YS Roque-Rosell, J Kim, C Cabana, J Kerr, J Kostecki, R AF Jarry, Angelique Gottis, Sebastien Yu, Young-Sang Roque-Rosell, Josep Kim, Chunjoong Cabana, Jordi Kerr, John Kostecki, Robert TI The Formation Mechanism of Fluorescent Metal Complexes at the LixNi0.5Mn1.5O4-delta/Carbonate Ester Electrolyte Interface SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID RECHARGEABLE LITHIUM BATTERIES; LI-ION BATTERIES; CATHODE MATERIALS; CHARGE-TRANSFER; OXIDE SURFACES; LINI0.5MN1.5O4; CHALLENGES; SPINEL; SPECTROSCOPY; PERFORMANCE AB Electrochemical oxidation of carbonate esters at the LixNi0.5Mn1.5O4-delta/electrolyte interface results in Ni/Mn dissolution and surface film formation, which negatively affect the electrochemical performance of Li-ion batteries. Ex situ X-ray absorption (XRF/XANES), Raman, and fluorescence spectroscopy, along with imaging of LixNi0.5Mn1.5O4-delta positive and graphite negative electrodes from tested Li-ion batteries, reveal the formation of a variety of Mn-II/III and Ni-II complexes with beta-diketonate ligands. These metal complexes, which are generated upon anodic oxidation of ethyl and diethyl carbonates at LixNi0.5Mn1.5O4-delta, form a surface film that partially dissolves in the electrolyte. The dissolved Mn-III complexes are reduced to their Mn-II analogues, which are incorporated into the solid electrolyte interphase surface layer at the graphite negative electrode. This work elucidates possible reaction pathways and evaluates their implications for Li+ transport kinetics in Li-ion batteries. C1 [Jarry, Angelique; Gottis, Sebastien; Kerr, John; Kostecki, Robert] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Yu, Young-Sang; Roque-Rosell, Josep] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Kim, Chunjoong; Cabana, Jordi] Univ Illinois, Dept Chem, Chicago, IL 60607 USA. RP Kostecki, R (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. EM r_kostecki@lbl.gov RI Roque Rosell, Josep/C-7868-2013; Cabana, Jordi/G-6548-2012 OI Roque Rosell, Josep/0000-0002-3518-1329; Cabana, Jordi/0000-0002-2353-5986 FU Energy Efficiency and Renewable Energy, Office of Vehicle Technologies, U.S. Department of Energy [DE-AC02-05CH11231]; Northeastern Center for Chemical Energy Storage, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001294]; Office of Science, Office of Basic Energy Sciences, U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies, U.S. Department of Energy, under Contract DE-AC02-05CH11231. Y.-S.Y. was supported by the Northeastern Center for Chemical Energy Storage, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award DE-SC0001294. Beamline 10.3.2 at the Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, U.S. Department of Energy under Contract DE-AC02-05CH11231. The authors thank Dr. Matthew Marcus (LBNL) for his help with the XANES experiments and data analysis. The authors also gratefully acknowledge Dr. Vincent S. Battaglia and Dr. Yanbao Fu (LBNL) for fruitful discussions and for supplying electrode materials. NR 47 TC 26 Z9 26 U1 20 U2 121 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAR 18 PY 2015 VL 137 IS 10 BP 3533 EP 3539 DI 10.1021/ja5116698 PG 7 WC Chemistry, Multidisciplinary SC Chemistry GA CD9LW UT WOS:000351420800021 PM 25714859 ER PT J AU Lee, K Kaseman, D Sen, S Hung, I Gan, ZH Gerke, B Pottgen, R Feygenson, M Neuefeind, J Lebedev, OI Kovnir, K AF Lee, Kathleen Kaseman, Derrick Sen, Sabyasachi Hung, Ivan Gan, Zhehong Gerke, Birgit Poettgen, Rainer Feygenson, Mikhail Neuefeind, Joerg Lebedev, Oleg I. Kovnir, Kirill TI Intricate Short-Range Ordering and Strongly Anisotropic Transport Properties of Li1-xSn2+xAs2 SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID LATTICE THERMAL-CONDUCTIVITY; CRYSTAL-STRUCTURE; PHONON-GLASS; THERMOELECTRIC-MATERIAL; HIGH-TEMPERATURE; ION BATTERIES; ZINTL-PHASES; LITHIUM; STANNIDES; SYSTEM AB A new ternary compound, Li1-xSn2+xAs2, 0.2 < x < 0.4, was synthesized via solid-state reaction of elements. The compound crystallizes in a layered structure in the R3 (_)m space group (No. 166) with SnAs layers separated by layers of jointly occupied Li/Sn atoms. The Sn-As layers are comprised of Sn3As3 puckered hexagons in a chair conformation that share all edges. Li/Sn atoms in the interlayer space are surrounded by a regular As-6 octahedron. Thorough investigation by synchrotron X-ray and neutron powder diffraction indicate no long-range Li/Sn ordering. In contrast, the local Li/Sn ordering was revealed by synergistic investigations via solid-state Li-6,Li-7 NMR spectroscopy, HRTEM, STEM, and neutron and X-ray pair distribution function analyses. Due to their different chemical natures, Li and Sn atoms tend to segregate into Li-rich and Sn-rich regions, creating substantial inhomogeneity on the nanoscale. The inhomogeneous local structure has a high impact on the physical properties of the synthesized compounds: the local Li/Sn ordering and multiple nanoscale interfaces result in unexpectedly low thermal conductivity and highly anisotropic resistivity in Li1-xSn2+xAs2. C1 [Lee, Kathleen; Kovnir, Kirill] Univ Calif Davis, Dept Chem, Davis, CA 95616 USA. [Kaseman, Derrick; Sen, Sabyasachi] Univ Calif Davis, Dept Chem Engn & Mat Sci, Davis, CA 95616 USA. [Hung, Ivan; Gan, Zhehong] Natl High Magnet Field Lab, Ctr Interdisciplinary Magnet Resonance, Tallahassee, FL 32310 USA. [Gerke, Birgit; Poettgen, Rainer] Univ Munster, Inst Anorgan & Analyt Chem, D-48149 Munster, Germany. [Feygenson, Mikhail; Neuefeind, Joerg] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. [Lebedev, Oleg I.] Univ Caen, Lab CRISMAT, ENSICAEN CNRS, UMR 6508, F-14050 Caen, France. RP Kovnir, K (reprint author), Univ Calif Davis, Dept Chem, One Shields Ave, Davis, CA 95616 USA. EM kkovnir@ucdavis.edu RI Neuefeind, Joerg/D-9990-2015; Feygenson, Mikhail /H-9972-2014; Gan, Zhehong/C-2400-2011 OI Neuefeind, Joerg/0000-0002-0563-1544; Feygenson, Mikhail /0000-0002-0316-3265; FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-SC0008931]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; National Science Foundation [DMR-0084173]; State of Florida FX This research is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, under Award No. DE-SC0008931. Use of the Advanced Photon Source at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. Research conducted at ORNL's Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. The National High Magnetic Field Laboratory is supported through the National Science Foundation Cooperative Agreement (DMR-0084173) and by the State of Florida. We thank Prof. S. M. Kauzlarich for access to the DSC. K.L. acknowledges the GAANN fellowship. NR 52 TC 5 Z9 5 U1 8 U2 76 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAR 18 PY 2015 VL 137 IS 10 BP 3622 EP 3630 DI 10.1021/jacs.5b00237 PG 9 WC Chemistry, Multidisciplinary SC Chemistry GA CD9LW UT WOS:000351420800032 PM 25702752 ER PT J AU Frost, SHL Frayo, SL Miller, BW Orozco, JJ Booth, GC Hylarides, MD Lin, YK Green, DJ Gopal, AK Pagel, JM Back, TA Fisher, DR Press, OW AF Frost, Sofia H. L. Frayo, Shani L. Miller, Brian W. Orozco, Johnnie J. Booth, Garrett C. Hylarides, Mark D. Lin, Yukang Green, Damian J. Gopal, Ajay K. Pagel, John M. Back, Tom A. Fisher, Darrell R. Press, Oliver W. TI Comparative Efficacy of Lu-177 and Y-90 for Anti-CD20 Pretargeted Radioimmunotherapy in Murine Lymphoma Xenograft Models SO PLOS ONE LA English DT Article ID B-CELL LYMPHOMAS; STREPTAVIDIN FUSION PROTEIN; NON-HODGKIN-LYMPHOMA; MONOCLONAL-ANTIBODY; PHASE I/II; INTRAPERITONEAL RADIOIMMUNOTHERAPY; OVARIAN-CANCER; MOUSE MODEL; THERAPY; TUMORS AB Purpose Pretargeted radioimmunotherapy (PRIT) is a multi-step method of selectively delivering high doses of radiotherapy to tumor cells while minimizing exposure to surrounding tissues. Yttrium-90 (Y-90) and lutetium-177 (Lu-177) are two of the most promising beta-particle emitting radionuclides used for radioimmunotherapy, which despite having similar chemistries differ distinctly in terms of radiophysical features. These differences may have important consequences for the absorbed dose to tumors and normal organs. Whereas Y-90 has been successfully applied in a number of preclinical and clinical radioimmunotherapy settings, there have been few published pretargeting studies with Lu-177. We therefore compared the therapeutic potential of targeting either Y-90 or Lu-177 to human B-cell lymphoma xenografts in mice. Methods Parallel experiments evaluating the biodistribution, imaging, dosimetry, therapeutic efficacy, and toxicity were performed in female athymic nude mice bearing either Ramos (Burkitt lymphoma) or Granta (mantle cell lymphoma) xenografts, utilizing an anti-CD20 antibody-streptavidin conjugate (1F5-SA) and an Y-90- or Lu-177-labeled 1,4,7,10-tetraazacyclododecane- 1,4,7,10-tetraacetic acid (DOTA)-biotin second step reagent. Results The two radionuclides displayed comparable biodistributions in tumors and normal organs; however, the absorbed radiation dose delivered to tumor was more than twice as high for Y-90 (1.3 Gy/MBq) as for Lu-177 (0.6 Gy/MBq). More importantly, therapy with Y-90-DOTA-biotin was dramatically more effective than with Lu-177-DOTA-biotin, with 100% of Ramos xenograft-bearing mice cured with 37 MBq Y-90, whereas 0% were cured using identical amounts of Lu-177-DOTA-biotin. Similar results were observed in mice bearing Granta xenografts, with 80% of the mice cured with Y-90-PRIT and 0% cured with 177Lu-PRIT. Toxicities were comparable with both isotopes. Conclusion Y-90 was therapeutically superior to 177Lu for streptavidin-biotin PRIT approaches in these human lymphoma xenograft models. C1 [Frost, Sofia H. L.; Frayo, Shani L.; Orozco, Johnnie J.; Booth, Garrett C.; Hylarides, Mark D.; Lin, Yukang; Green, Damian J.; Gopal, Ajay K.; Pagel, John M.; Press, Oliver W.] Fred Hutchinson Canc Res Ctr, Div Clin Res, Seattle, WA 98104 USA. [Miller, Brian W.] Pacific Northwest Natl Lab, Richland, WA USA. [Miller, Brian W.] Univ Arizona, Coll Opt Sci, Tucson, AZ USA. [Green, Damian J.; Gopal, Ajay K.; Pagel, John M.; Press, Oliver W.] Univ Washington, Dept Med, Seattle, WA USA. [Green, Damian J.; Gopal, Ajay K.; Pagel, John M.; Press, Oliver W.] Univ Washington, Dept Bioengn, Seattle, WA 98195 USA. [Back, Tom A.] Univ Gothenburg, Sahlgrenska Acad, Gothenburg, Sweden. [Fisher, Darrell R.] Dade Moeller Hlth Grp, Richland, WA USA. RP Frost, SHL (reprint author), Fred Hutchinson Canc Res Ctr, Div Clin Res, 1124 Columbia St, Seattle, WA 98104 USA. EM sfrost@fredhutch.org OI Back, Tom/0000-0002-3375-9473 FU Walker Immunotherapy Research Fellowship from Doug and Maggie Walker; David & Patricia Giuliani Family Foundation; Geoffrey Sally White; Wyner-Stokes Foundation; Frederick Kullman Memorial Fund; National Cancer Institute [P01CA044991, R01CA076287, R01CA138720, R01CA172582, R01CA136639, R01CA154897, R01CA109663, K08CA151682]; Dade Moeller Health Group FX Research reported in this manuscript was supported by a Walker Immunotherapy Research Fellowship from Doug and Maggie Walker (SHLF); by the David & Patricia Giuliani Family Foundation (OWP); by Geoffrey & Sally White (OWP); by the Wyner-Stokes Foundation (OWP); by the Frederick Kullman Memorial Fund (JMP); and by the National Cancer Institute under award numbers P01CA044991 (OWP, MDH, YL, AKG, JMP, DRF), R01CA076287 (OWP, SLF, GCB, MDH, YL, JMP), R01CA138720 (JMP, JJO), R01CA172582 (JMP), R01CA136639 (OWP, YL), R01CA154897 (OWP, DJG), R01CA109663 (OWP, SLF, GCB, MDH, YL, JMP), and K08CA151682 (DJG). Dade Moeller Health Group provided support in the form of salary for author DRF, but did not have any additional role in the study design, data collection and analysis, decision to publish, or preparation of the manuscript. The specific role of this author is articulated in the 'author contributions' section. NR 40 TC 2 Z9 2 U1 4 U2 16 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAR 18 PY 2015 VL 10 IS 3 AR e0120561 DI 10.1371/journal.pone.0120561 PG 16 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CE9BN UT WOS:000352138500181 PM 25785845 ER PT J AU VanDelinder, V Wheeler, DR Small, LJ Brumbach, MT Spoerke, ED Henderson, I Bachand, GD AF VanDelinder, Virginia Wheeler, David R. Small, Leo J. Brumbach, Michael T. Spoerke, Erik D. Henderson, Ian Bachand, George D. TI Simple, Benign, Aqueous-Based Amination of Polycarbonate Surfaces SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE polycarbonate; aminated surface; surface chemistry; bacteriorhodopsin; antibiofoulin; functionalized surface ID COVALENT IMMOBILIZATION; PROTEIN LIGAND; COMPACT DISC; ACTIVATION; MEMBRANE; OXYGEN; XPS AB Polycarbonate is a desirable material for many applications due to its favorable mechanical and optical properties. Here, we report a simple, safe, environmentally friendly aqueous method that uses diamines to functionalize a polycarbonate surface with amino groups. The use of water as the solvent for the functionalization ensures that solvent induced swelling does not affect the optical or mechanical properties of the polycarbonate. We characterize the efficacy of the surface amination using X-ray photo spectroscopy, Fourier transform infrared spectroscopy (FT-IR), atomic force microscopy (AFM), and contact angle measurements. Furthermore, we demonstrate the ability of this facile method to serve as a foundation upon which other functionalities may be attached, including antifouling coatings and oriented membrane proteins. C1 [VanDelinder, Virginia; Henderson, Ian; Bachand, George D.] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87111 USA. [Wheeler, David R.] Sandia Natl Labs, Biosensors & Nanomat, Albuquerque, NM 87111 USA. [Small, Leo J.; Spoerke, Erik D.] Sandia Natl Labs, Elect Opt & Nano Mat, Albuquerque, NM 87111 USA. [Brumbach, Michael T.] Sandia Natl Labs, Mat Characterizat & Performance, Albuquerque, NM 87111 USA. RP Wheeler, DR (reprint author), Sandia Natl Labs, Biosensors & Nanomat, POB 5800,MS 1141, Albuquerque, NM 87111 USA. EM drwheel@sandia.gov; gdbacha@sandia.gov OI Small, Leo/0000-0003-0404-6287; Bachand, George/0000-0002-3169-9980 FU U.S. Department of Energy (DOE) Office of Science [U2013A0096]; Sandia National Laboratories' Laboratory Directed Research and Development program [165696]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work, in part, was performed at the Center for Integrated Nanotechnologies (user project U2013A0096), an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science. This work was supported by Sandia National Laboratories' Laboratory Directed Research and Development program (project 165696). Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 25 TC 5 Z9 5 U1 9 U2 24 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD MAR 18 PY 2015 VL 7 IS 10 BP 5643 EP 5649 DI 10.1021/am508797h PG 7 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA CD9LR UT WOS:000351420300005 PM 25695347 ER PT J AU Wu, HC Kessler, MR AF Wu, Hongchao Kessler, Michael R. TI Multifunctional Cyanate Ester Nanocomposites Reinforced by Hexagonal Boron Nitride after Noncovalent Biomimetic Functionalization SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE boron nitride; polymer matrix composites (PMCs); surface functionalization; thermo-mechanical properties; dielectric properties; thermal conductivity ID THERMAL-CONDUCTIVITY IMPROVEMENT; MECHANICAL-PROPERTIES; EPOXY COMPOSITES; ELECTRONIC ENCAPSULATION; POLYMER NANOCOMPOSITES; SURFACE MODIFICATION; CARBON NANOTUBES; FILMS; PERFORMANCE; DOPAMINE AB Boron nitride (BN) reinforced polymer nanocomposites have attracted a growing research interest in the microelectronic industry for their uniquely thermal conductive but electrical insulating properties. To overcome the challenges in surface functionalization, in this study, hexagonal boron nitride (h-BN) nanopartides were noncovalently modified with polydopamine in a solvent-free aqueous condition. The strong pi-pi interaction between the hexagonal structural BN and aromatic dopamine molecules facilitated 15 wt % polydopamine encapsulating the nanopartides. High-performance bisphenol E cyanate ester (BECy) was incorporated by homogeneously dispersed h-BN at different loadings and functionalities to investigate their effects on thermomechanical, dynamic-mechanical, and dielectric properties, as well as thermal conductivity. Different theoretical and empirical models were successfully applied to predict thermal and dielectric properties of h-BN/BECy nanocomposites. Overall, the prepared h-BN/BECy nanocomposites exhibited outstanding performance in dimensional stability, dynamic-mechanical properties, and thermal conductivity, together with the controllable dielectric property and preserved thermal stability for high-temperature applications. C1 [Wu, Hongchao; Kessler, Michael R.] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. [Kessler, Michael R.] US DOE, Ames Lab, Ames, IA 50011 USA. [Kessler, Michael R.] Washington State Univ, Sch Mech & Mat Engn, Pullman, WA 99164 USA. RP Kessler, MR (reprint author), Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. EM MichaelR.Kessler@wsu.edu RI Kessler, Michael/C-3153-2008; Wu, Hongchao/D-4808-2016 OI Kessler, Michael/0000-0001-8436-3447; Wu, Hongchao/0000-0002-0195-8398 FU Honeywell Federal Manufacturing & Technologies, LLC; Air Force Office of Scientific Research [FA9550-12-1-0108] FX The authors acknowledge partial funding for this project by Honeywell Federal Manufacturing & Technologies, LLC and the Air Force Office of Scientific Research (Award No. FA9550-12-1-0108). The authors also acknolwedge Tacey Pepper (Genetics, Development & Cell Biology, Iowa State University) for her assitance with TEM measurement, and Landi Zhong (Materials Science and Engieering, Iowa State University) for the thermal conductivity measurement. NR 61 TC 21 Z9 22 U1 22 U2 133 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD MAR 18 PY 2015 VL 7 IS 10 BP 5915 EP 5926 DI 10.1021/acsami.5b00147 PG 12 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA CD9LR UT WOS:000351420300035 PM 25726956 ER PT J AU Hu, YX Liu, YZ Sun, YG AF Hu, Yongxing Liu, Yuzi Sun, Yugang TI Mesoporous Colloidal Superparticles of Platinum-Group Nanocrystals with Surfactant-Free Surfaces and Enhanced Heterogeneous Catalysis SO ADVANCED FUNCTIONAL MATERIALS LA English DT Article ID SEMICONDUCTOR NANORODS; NANOPARTICLE CLUSTERS; ACTIVATION-ENERGY; COPOLYMERS; METALS; GROWTH; FILMS; GOLD AB Synthesis of colloidal superparticles (CSPs) of nanocrystals, a class of assembled nanocrystals in the form of colloidal particles, has been emerging as a new frontier in the field of nanotechnology because of their potential novel properties originated from coupling of individual nanocrystals in CSPs. Here, a facile approach is reported for the controlled synthesis of mesoporous CSPs made of various platinum-group nanocrystals that exhibit high colloidal stability and ligand-free surfaces to significantly benefit their applications in solution-phase heterogeneous catalysis. The synthesis relies on self-limiting growth of composite particles through coprecipitation of both Pt-group nanocrystals (or their precursor compounds) and silver halides on sacrificial substrates of colloidal silver particles. The intermediate silver halides in the composite particles play the critical role in limiting the continuous growth (and/or coalescence) of individual Pt-group nanocrystals and they can be selectively dissolved to create nanoscale pores in the resulting CSPs. C1 [Hu, Yongxing; Liu, Yuzi; Sun, Yugang] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. RP Hu, YX (reprint author), Argonne Natl Lab, Ctr Nanoscale Mat, 9700 S Cass Ave, Argonne, IL 60439 USA. EM ygsun@anl.gov RI Sun, Yugang /A-3683-2010; Liu, Yuzi/C-6849-2011 OI Sun, Yugang /0000-0001-6351-6977; FU Center for Nanoscale Materials, a U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility [DE-AC02-06CH11357] FX This work was performed at the Center for Nanoscale Materials, a U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility under Contract No. DE-AC02-06CH11357. The authors thank Dr. Zheng Li for help. NR 38 TC 7 Z9 7 U1 9 U2 79 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1616-301X EI 1616-3028 J9 ADV FUNCT MATER JI Adv. Funct. Mater. PD MAR 18 PY 2015 VL 25 IS 11 BP 1638 EP 1647 DI 10.1002/adfm.201403664 PG 10 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CD6QL UT WOS:000351214000002 ER PT J AU Xu, M Ilton, ES Engelhard, MH Qafoku, O Felmy, AR Rosso, KM Kerisit, S AF Xu, Man Ilton, Eugene S. Engelhard, Mark H. Qafoku, Odeta Felmy, Andrew R. Rosso, Kevin M. Kerisit, Sebastien TI Heterogeneous growth of cadmium and cobalt carbonate phases at the (10(1)over-bar4) calcite surface SO CHEMICAL GEOLOGY LA English DT Article DE Metal carbonates; Nucleation and growth; Heteroepitaxy; Lattice misfit ID X-RAY PHOTOELECTRON; SOLID-SOLUTION FORMATION; WATER-EXCHANGE; AQUEOUS-SOLUTIONS; METAL-IONS; IN-SITU; HETEROEPITAXIAL GROWTH; SPECTROSCOPIC XPS; EPITAXIAL-GROWTH; FREE-ENERGY AB The ability of surface precipitates to form heteroepitaxially is an important factor that controls the extent of heterogeneous growth. In this work, the growth of cadmium and cobalt carbonate phases on (10 (1) over bar4 ) calcite surfaces is compared for a range of initial saturation states with respect to otavite (CdCO3) and sphaerocobaltite (CoCO3), two isostructural metal carbonates that exhibit different lattice misfits with respect to calcite (-4% and -15%, respectively, based on (10 (1) over bar4) surface areas). Calcite single crystals were reacted in static conditions for 16 h with CdCl2 and CoCl2 aqueous solutions with initial concentrations 0.3 <= [ Cd2+](0) <= 100 mu M and 25 <= [ Co2+](0) <= 200 mu M. The reacted crystals were imaged in situ with atomic force microscopy (AFM) and analyzed ex situ with X-ray photoelectron spectroscopy (XPS). AFM images of Cd-reacted crystals showed the formation of large islands elongated along the [42 (1) over bar] direction, clear evidence of heteroepitaxial growth, whereas surface precipitates on Co-reacted crystals were small round islands. Deformation of calcite etch pits in both cases indicated the incorporation of Cd and Co at step edges. XPS analysis pointed to the formation of a Cd-rich (Ca, Cd)CO3 solid solution coating atop the calcite substrate. In contrast, XPS measurements of the Co-reacted crystals provided evidence for the formation of a mixed hydroxy-carbonate cobalt phase despite supersaturation with respect to CoCO3. The combined AFM and XPS results suggest that the lattice misfit between CoCO3 and CaCO3 is too large to allow for heteroepitaxial growth of a pure cobalt carbonate phase on calcite surfaces in aqueous solutions and at ambient conditions. The use of the satellite structure of the Co 2p(3/2) photoelectron line as a tool for determining the nature of cobalt surface precipitates is also discussed. (C) 2015 Elsevier B.V. All rights reserved.The ability of surface precipitates to form heteroepitaxially is an important factor that controls the extent of heterogeneous growth. In this work, the growth of cadmium and cobalt carbonate phases on (10 (1) over bar4 ) calcite surfaces is compared for a range of initial saturation states with respect to otavite (CdCO3) and sphaerocobaltite (CoCO3), two isostructural metal carbonates that exhibit different lattice misfits with respect to calcite (-4% and -15%, respectively, based on (10 (1) over bar4) surface areas). Calcite single crystals were reacted in static conditions for 16 h with CdCl2 and CoCl2 aqueous solutions with initial concentrations 0.3 <= [ Cd2+](0) <= 100 mu M and 25 <= [ Co2+](0) <= 200 mu M. The reacted crystals were imaged in situ with atomic force microscopy (AFM) and analyzed ex situ with X-ray photoelectron spectroscopy (XPS). AFM images of Cd-reacted crystals showed the formation of large islands elongated along the [42 (1) over bar] direction, clear evidence of heteroepitaxial growth, whereas surface precipitates on Co-reacted crystals were small round islands. Deformation of calcite etch pits in both cases indicated the incorporation of Cd and Co at step edges. XPS analysis pointed to the formation of a Cd-rich (Ca, Cd)CO3 solid solution coating atop the calcite substrate. In contrast, XPS measurements of the Co-reacted crystals provided evidence for the formation of a mixed hydroxy-carbonate cobalt phase despite supersaturation with respect to CoCO3. The combined AFM and XPS results suggest that the lattice misfit between CoCO3 and CaCO3 is too large to allow for heteroepitaxial growth of a pure cobalt carbonate phase on calcite surfaces in aqueous solutions and at ambient conditions. The use of the satellite structure of the Co 2p(3/2) photoelectron line as a tool for determining the nature of cobalt surface precipitates is also discussed. (C) 2015 Elsevier B.V. All rights reserved. C1 [Xu, Man; Ilton, Eugene S.; Qafoku, Odeta; Felmy, Andrew R.; Rosso, Kevin M.; Kerisit, Sebastien] Pacific NW Natl Lab, Div Phys Sci, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. [Engelhard, Mark H.] Pacific NW Natl Lab, Sci Resources Div, Environm Mol Sci Lab, Richland, WA 99352 USA. RP Kerisit, S (reprint author), Pacific NW Natl Lab, Div Phys Sci, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. EM sebastien.kerisit@pnnl.gov FU Geosciences Research Program of the U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences Biosciences; U.S. DOE's Office of Biological and Environmental Research; DOE by Battelle Memorial Institute [DE-AC06-76RLO-1830] FX This work was supported by the Geosciences Research Program of the U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences & Biosciences. The research was performed using the Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by the U.S. DOE's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory (PNNL). PNNL is operated for DOE by Battelle Memorial Institute under Contract# DE-AC06-76RLO-1830. The authors acknowledge Mark Bowden for the mu-XRD characterization of the synthesized CoCO3 powder sample. NR 64 TC 1 Z9 1 U1 6 U2 37 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2541 EI 1878-5999 J9 CHEM GEOL JI Chem. Geol. PD MAR 18 PY 2015 VL 397 BP 24 EP 36 DI 10.1016/j.chemgeo.2015.01.003 PG 13 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA CE2TP UT WOS:000351671900003 ER PT J AU Anastasiou, C Duhr, C Dulat, F Furlan, E Gehrmann, T Herzog, F Mistlberger, B AF Anastasiou, Charalampos Duhr, Claude Dulat, Falko Furlan, Elisabetta Gehrmann, Thomas Herzog, Franz Mistlberger, Bernhard TI Higgs boson gluon-fusion production beyond threshold in (NLO)-L-3 QCD SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE QCD Phenomenology; NLO Computations ID 3-LOOP SPLITTING FUNCTIONS; BETA-FUNCTION; ANOMALOUS DIMENSIONS; PROTON COLLIDERS; HADRON COLLIDERS; LEPTON-PAIR; NNLO; LHC AB In this article, we compute the gluon fusion Higgs boson cross-section at (NLO)-L-3 through the second term in the threshold expansion. This calculation constitutes a major milestone towards the full (NLO)-L-3 cross section. Our result has the best formal accuracy in the threshold expansion currently available, and includes contributions from collinear regions besides subleading corrections from soft and hard regions, as well as certain logarithmically enhanced contributions for general kinematics. We use our results to perform a critical appraisal of the validity of the threshold approximation at (NLO)-L-3 in perturbative QCD. C1 [Anastasiou, Charalampos; Dulat, Falko; Mistlberger, Bernhard] ETH, Inst Theoret Phys, CH-8093 Zurich, Switzerland. [Duhr, Claude] Catholic Univ Louvain, Ctr Cosmol Particle Phys & Phenomenol CP3, B-1348 Louvain, Belgium. [Furlan, Elisabetta] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Gehrmann, Thomas] Univ Zurich, Inst Phys, CH-8057 Zurich, Switzerland. [Herzog, Franz] Nikhef, NL-1098 XG Amsterdam, Netherlands. [Herzog, Franz] CERN, Div Theory, CH-1211 Geneva 23, Switzerland. RP Anastasiou, C (reprint author), ETH, Inst Theoret Phys, CH-8093 Zurich, Switzerland. EM babis@ethz.ch; claude.duhr@uclouvain.be; dulatf@itp.phys.ethz.ch; efurlan@fnal.gov; thomas.gehrmann@uzh.ch; franz.herzog@cern.ch; bmistlbe@itp.phys.ethz.ch RI Gehrmann, Thomas/J-4940-2016; OI Gehrmann, Thomas/0000-0001-7009-432X; Furlan, Elisabetta/0000-0001-7036-9012 FU Swiss National Science Foundation (SNF) [200021-143781, 200020-149517]; European Commission through the ERC [291377, 320651, 340983]; FP7 Marie Curie Initial Training Network "LHCPhenoNet" [PITN-GA-2010264564]; U.S. Department of Energy [DE-AC02-07CH11359]; Fonds National de la Recherche Scientifique (FNRS), Belgium FX The authors are grateful to Achilleas Lazopoulos and Andreas Vogt for discussions. This research was supported by the Swiss National Science Foundation (SNF) under contracts 200021-143781 and 200020-149517, the European Commission through the ERC grants "IterQCD", "LHCTheory" (291377), "HEPGAME" (320651) and "MC@NNLO" (340983) and the FP7 Marie Curie Initial Training Network "LHCPhenoNet" (PITN-GA-2010264564), by the U.S. Department of Energy under contract no. DE-AC02-07CH11359 and the "Fonds National de la Recherche Scientifique" (FNRS), Belgium. NR 55 TC 17 Z9 17 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAR 18 PY 2015 IS 3 AR 091 DI 10.1007/JHEP03(2015)091 PG 25 WC Physics, Particles & Fields SC Physics GA CD8TY UT WOS:000351370300003 ER PT J AU Yan, HJ Chuang, C Zhugayevych, A Tretiak, S Dahlquist, FW Bazan, GC AF Yan, Hengjing Chuang, Chern Zhugayevych, Andriy Tretiak, Sergei Dahlquist, Frederick W. Bazan, Guillermo C. TI Inter-Aromatic Distances in Geobacter Sulfurreducens Pili Relevant to Biofilm Charge Transport SO ADVANCED MATERIALS LA English DT Article ID MOLECULAR-ORBITAL METHODS; SWISS-MODEL WORKSPACE; GAUSSIAN-TYPE BASIS; ORGANIC SEMICONDUCTORS; ELECTRICAL-CONDUCTIVITY; MICROBIAL NANOWIRES; CARRIER TRANSPORT; PENTACENE; SIMULATION; PARAMETERS AB Geobacter sulfurreducens pili are implicated in facilitating electron transfer to electrode surfaces. Comparisons are made between the conductivity of pili and that of doped organic semi conductors, invoking mechanisms such as "electron hopping" or "metallic conduction". Analysis of inter-aromatic distances in these pili models shows that charge-carrier transport involving only the pi-conjugated system of GS pili is negligible. C1 [Yan, Hengjing] Univ Calif Santa Barbara, Ctr Polymers & Organ Solids, Dept Chem & Biochem, Santa Barbara, CA 93106 USA. [Chuang, Chern; Zhugayevych, Andriy; Tretiak, Sergei] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Dahlquist, Frederick W.] Univ Calif Santa Barbara, Dept Mol Cellular & Dev Biol, Dept Chem & Biochem, Santa Barbara, CA 93106 USA. [Bazan, Guillermo C.] Univ Calif Santa Barbara, Dept Mat, Dept Chem & Biochem, Ctr Polymers & Organ Solids, Santa Barbara, CA 93106 USA. RP Tretiak, S (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM serg@lanl.gov; dahlquist@chem.ucsb.edu; bazan@chem.ucsb.edu RI Tretiak, Sergei/B-5556-2009; Bazan, Guillermo/B-7625-2014 OI Tretiak, Sergei/0000-0001-5547-3647; FU Institute for Collaborative Biotechnologies (ICB) from U.S. Army Research Office [W911F-09-D-0001]; LANL LDRD program; Center for Integrated Nanotechnologies, a U.S. Department of Energy FX Funding was provided by the Institute for Collaborative Biotechnologies (ICB) under Grant No. W911F-09-D-0001 from the U.S. Army Research Office. This work was partially supported by LANL LDRD program and the Center for Integrated Nanotechnologies, a U.S. Department of Energy, and the Office of Basic Energy Sciences user facility. NR 31 TC 9 Z9 9 U1 7 U2 37 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD MAR 18 PY 2015 VL 27 IS 11 BP 1908 EP + DI 10.1002/adma.201404167 PG 5 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CD6RJ UT WOS:000351216500013 PM 25604785 ER PT J AU Chen, B Laverock, J Newby, D McNulty, JF Smith, KE Glans, PA Guo, JH Qiao, RM Yang, WL Lees, MR Tung, LD Singh, RP Balakrishnan, G AF Chen, B. Laverock, J. Newby, D., Jr. McNulty, J. F. Smith, K. E. Glans, P-A Guo, J-H Qiao, R-M Yang, W-L Lees, M. R. Tung, L. D. Singh, R. P. Balakrishnan, G. TI Effects of rare-earth size on the electronic structure of La1-xLuxVO3 SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE x-ray absorption spectra; x-ray emission spectra and fluorescence; resonant inelastic x-ray scattering; local spin density approximation; electron density of states; strongly correlated electron systems ID TRANSITION-METAL OXIDES; RAY; SPECTROSCOPY; DIFFRACTION; SPECTRA; EVOLUTION AB The electronic structure of La1-xLuxVO3(x = 0, 0.2, 0.6 and 1) single crystals has been investigated using soft x-ray absorption spectroscopy, soft x-ray emission spectroscopy, and resonant soft x-ray inelastic scattering to study the effects of rare-earth size. The x-ray absorption and emission spectra at the O K-edge present a progressive evolution with R-site cation, in agreement with local spin density approximation calculations. This evolution with R, together with the temperature dependence of the O K-edge spectra, is attributed to changes in the crystal structure of La1-xLuxVO3. The crystal-field dd* excitations probed by resonant inelastic x-ray scattering at the V L3-edge exhibit an increase in energy and enhanced intensity with the decrease of R-site ionic radius, which is mainly attributed to the increased tilting magnitude of the VO6 octahedra. Upon cooling to similar to 95 K, the dd* excitations are prominently enhanced in relative intensity, in agreement with the formation of the Jahn-Teller distortion in the orbital ordering phase. Additionally, the dd* transitions of the mixed compounds are noticeably suppressed with respect to those of the pure compounds, possibly owing to the formation of C-type orbital ordering induced by large R-site size variances. C1 [Chen, B.; Laverock, J.; Newby, D., Jr.; McNulty, J. F.; Smith, K. E.] Boston Univ, Dept Phys, Boston, MA 02215 USA. [Glans, P-A; Guo, J-H; Qiao, R-M; Yang, W-L] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Lees, M. R.; Tung, L. D.; Singh, R. P.; Balakrishnan, G.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Smith, K. E.] Univ Auckland, Sch Chem Sci, Auckland 1142, New Zealand. [Smith, K. E.] Univ Auckland, MacDiarmid Inst Adv Mat & Nanotechnol, Auckland 1142, New Zealand. RP Chen, B (reprint author), Boston Univ, Dept Phys, 590 Commonwealth Ave, Boston, MA 02215 USA. EM bchen727@bu.edu RI Laverock, Jude/G-4537-2010; Qiao, Ruimin/E-9023-2013; Yang, Wanli/D-7183-2011; Lees, Martin/D-9584-2013; Glans, Per-Anders/G-8674-2016; Balakrishnan, Geetha/P-5977-2016; Chen, Bo/C-5428-2017 OI Laverock, Jude/0000-0003-3653-8171; Yang, Wanli/0000-0003-0666-8063; Lees, Martin/0000-0002-2270-2295; Balakrishnan, Geetha/0000-0002-5890-1149; Chen, Bo/0000-0002-9263-5171 FU Department of Energy [DE-FG02-98ER45680]; Director, Office of Science, Office of Basic Energy Sciences, of the US Department of Energy [DE-AC02-05CH11231]; EPSRC [EP/I007210/1]; Boston University/University of Warwick collaboration fund FX The Boston University program is supported by the Department of Energy under Grant No. DE-FG02-98ER45680. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the US Department of Energy under Contract No. DE-AC02-05CH11231. GB gratefully acknowledges financial support from EPSRC Grant EP/I007210/1. This project is also supported in part by the Boston University/University of Warwick collaboration fund. NR 48 TC 2 Z9 2 U1 1 U2 22 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD MAR 18 PY 2015 VL 27 IS 10 AR 105503 DI 10.1088/0953-8984/27/10/105503 PG 13 WC Physics, Condensed Matter SC Physics GA CB8QL UT WOS:000349895700010 PM 25710627 ER PT J AU Fan, XF Zheng, WT Kuo, JL Singh, DJ AF Fan, Xiaofeng Zheng, W. T. Kuo, Jer-Lai Singh, David J. TI Structural stability of single-layer MoS2 under large strain SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE soft phonon mode; first-principle calculation; MoS2 ID TRANSITION-METAL DICHALCOGENIDES; TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; MONOLAYER MOS2; TRANSISTORS AB Out-of-plane relaxation can introduce MoS2 in flexible electronic/optoelectronic devices, while under larger strain it is possible to frustrate the structure of MoS2. On the basis of first-principle calculations, the ideal tensile stress strain relations and failure mechanism of single-layer MoS2 structure under large strain is investigated. The instability of phonon modes near the K point results in the decrease of tensile stress under large strain. The relative out-of-plane movement of Mo atoms is found to contribute to the mechanism of the soft phonon mode. C1 [Fan, Xiaofeng; Zheng, W. T.; Singh, David J.] Jilin Univ, Coll Mat Sci & Engn, Changchun 130012, Peoples R China. [Kuo, Jer-Lai] Acad Sinica, Inst Atom & Mol Sci, Taipei 10617, Taiwan. [Singh, David J.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Fan, XF (reprint author), Jilin Univ, Coll Mat Sci & Engn, Changchun 130012, Peoples R China. EM xffan@jlu.edu.cn; singhdj@ornl.gov RI Fan, Xiaofeng/B-9680-2011; Kuo, Jer-Lai/F-5689-2010 OI Fan, Xiaofeng/0000-0001-6288-4866; NR 29 TC 7 Z9 7 U1 10 U2 74 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD MAR 18 PY 2015 VL 27 IS 10 AR 105401 DI 10.1088/0953-8984/27/10/105401 PG 5 WC Physics, Condensed Matter SC Physics GA CB8QL UT WOS:000349895700007 PM 25706676 ER PT J AU Uervirojnangkoorn, M Zeldin, OB Lyubimov, AY Hattne, J Brewster, AS Sauter, NK Brunger, AT Weis, WI AF Uervirojnangkoorn, Monarin Zeldin, Oliver B. Lyubimov, Artem Y. Hattne, Johan Brewster, Aaron S. Sauter, Nicholas K. Brunger, Axel T. Weis, William I. TI Enabling X-ray Free Electron Laser Crystallography for Challenging Biological Systems from a Limited Number of Crystals SO ELIFE LA English DT Article DE structural biology; light sources; X-ray free electron laser; post-refinement ID SERIAL FEMTOSECOND CRYSTALLOGRAPHY; MACROMOLECULAR CRYSTALLOGRAPHY; PROTEIN CRYSTALS; PYTHON; XFEL; REFINEMENT; RADIATION; SOFTWARE; QUALITY; DAMAGE C1 [Uervirojnangkoorn, Monarin; Zeldin, Oliver B.; Lyubimov, Artem Y.; Brunger, Axel T.; Weis, William I.] Stanford Univ, Dept Cellular & Mol Physiol, Stanford, CA 94305 USA. [Uervirojnangkoorn, Monarin; Zeldin, Oliver B.; Lyubimov, Artem Y.; Brunger, Axel T.] Stanford Univ, Dept Neurol & Neurol Sci, Stanford, CA 94305 USA. [Uervirojnangkoorn, Monarin; Zeldin, Oliver B.; Lyubimov, Artem Y.; Brunger, Axel T.] Stanford Univ, Dept Structural Biol, Stanford, CA 94305 USA. [Uervirojnangkoorn, Monarin; Zeldin, Oliver B.; Lyubimov, Artem Y.; Brunger, Axel T.; Weis, William I.] Stanford Univ, Dept Photon Sci, Stanford, CA 94305 USA. [Uervirojnangkoorn, Monarin; Zeldin, Oliver B.; Lyubimov, Artem Y.; Brunger, Axel T.] Stanford Univ, Howard Hughes Med Inst, Stanford, CA 94305 USA. [Brewster, Aaron S.; Sauter, Nicholas K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Brunger, AT (reprint author), Stanford Univ, Dept Cellular & Mol Physiol, Stanford, CA 94305 USA. EM brunger@stanford.edu; bill.weis@stanford.edu RI Sauter, Nicholas/K-3430-2012; Weis, William/G-1437-2011; OI Weis, William/0000-0002-5583-6150; Brunger, Axel/0000-0001-5121-2036; Hattne, Johan/0000-0002-8936-0912 FU National Institutes of Health [GM095887, GM102520]; Office of Science, Department of Energy [DE-AC02-05CH11231]; HHMI Collaborative Innovation Award (HCIA) FX We thank Henrik Lemke, Sebastien Boutet, and Ralf Grosse-Kunstleve for discussions. We thank S. Michael Soltis, Aina E. Cohen, Ana Gonzalez, Yingssu Tsai, Winnie Brehmer, Laura Aguila, Jinhu Song, Scott McPhillips and Henrik Lemke for providing the XFEL diffraction data sets of myoglobin. We thank John W. Peters, Stephen Keable, Oleg A. Zadvornyy, Aina E. Cohen, S. Michael Soltis, Jinhu Song, Scott McPhillips, Clyde Smith and Henrik Lemke for providing the XFEL diffraction data sets of Cpl hydrogenase, and the Lawrence Berkeley National Laboratory for providing computational resources. Portions of this research were carried out at the Linac Coherent Light Source (LCLS) at the SLAC National Accelerator Laboratory. LCLS is an Office of Science User Facility operated for the U.S. Department of Energy Office of Science by Stanford University. A.S.B. and N.K.S. were supported by National Institutes of Health grants GM095887 and GM102520 and Director, Office of Science, Department of Energy under contract DE-AC02-05CH11231. This work is supported by a HHMI Collaborative Innovation Award (HCIA) to A.T.B. and W.I.W. NR 39 TC 21 Z9 22 U1 0 U2 6 PU ELIFE SCIENCES PUBLICATIONS LTD PI CAMBRIDGE PA SHERATON HOUSE, CASTLE PARK, CAMBRIDGE, CB3 0AX, ENGLAND SN 2050-084X J9 ELIFE JI eLife PD MAR 17 PY 2015 VL 4 AR e05421 DI 10.7554/eLife.05421 PG 69 WC Biology SC Life Sciences & Biomedicine - Other Topics GA CE5IQ UT WOS:000351865600006 ER PT J AU Kim, S Guenther, A Lefer, B Flynn, J Griffin, R Rutter, AP Gong, LW Cevik, BK AF Kim, Saewung Guenther, Alex Lefer, Barry Flynn, James Griffin, Robert Rutter, Andrew P. Gong, Longwen Cevik, Basak Karakurt TI Potential Role of Stabilized Criegee Radicals in Sulfuric Acid Production in a High Biogenic VOC Environment SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID VOLATILE ORGANIC-COMPOUNDS; MASTER CHEMICAL MECHANISM; MCM V3 PART; TROPOSPHERIC DEGRADATION; GAS-PHASE; ATMOSPHERIC OXIDATION; DIOXIDE OXIDATION; INTERMEDIATE; SO2; OZONE AB We present field observations made in June 2011 downwind of Dallas Fort Worth, TX, and evaluate the role of stabilized Criegee radicals (sCIs) in gaseous sulfuric acid (H2SO4) production. Zero-dimensional model calculations show that sCI from biogenic volatile organic compounds composed the majority of the sCIs. The main uncertainty associated with an evaluation of H2SO4 production from the sCI reaction channel is the lack of experimentally determined reaction rates for sCIs formed from isoprene ozonolysis with 502 along with systematic discrepancies in experimentally derived reaction rates between other sCIs and SO2 and water vapor. In general, the maximum of H2SO4 production from the sCI channel is found in the late afternoon as ozone increases toward the late afternoon. The sCI channel, however, contributes minor H2SO4 production compared with the conventional OH channel in the mid-day. Finally, the production and the loss rates of H2SO4 are compared. The application of the recommended mass accommodation coefficient causes significant overestimation of H2SO4 loss rates compared with H2SO4 production rates. However, the application of a lower experimental value for the mass accommodation coefficient provides good agreement between the loss and production rates of H2SO4. The results suggest that the recommended coefficient for the H2O surface may not be suitable for this relatively dry environment. C1 [Kim, Saewung] Univ Calif Irvine, Dept Earth Syst Sci, Irvine, CA 92697 USA. [Guenther, Alex] Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99354 USA. [Guenther, Alex] Washington State Univ, Dept Civil & Environm Engn, Pullman, WA 99164 USA. [Lefer, Barry; Flynn, James] Univ Houston, Dept Earth & Atmospher Sci, Houston, TX 77004 USA. [Griffin, Robert; Rutter, Andrew P.; Gong, Longwen; Cevik, Basak Karakurt] Rice Univ, Dept Civil & Environm Engn, Houston, TX 77005 USA. [Rutter, Andrew P.] SC Johnson & Son Inc, Racine, WI 53403 USA. [Gong, Longwen] Calif Air Resource Board, Monitoring & Lab Div, Sacramento, CA 95811 USA. RP Kim, S (reprint author), Univ Calif Irvine, Dept Earth Syst Sci, Irvine, CA 92697 USA. EM saewungk@uci.edu RI Kim, Saewung/E-4089-2012; OI Lefer, Barry/0000-0001-9520-5495 FU TCEQ Air Quality Research Program; Dreyfus Foundation FX This study was supported by the TCEQ Air Quality Research Program. Support of A.P. Rutter by the Dreyfus Foundation is gratefully acknowledged. The authors would like to thank Melanie Calzada and Caroline Gutierrez for their help in data collection in the field and the Texas National Guard for providing access to the Eagle Mountain Lake site. NR 49 TC 4 Z9 4 U1 13 U2 66 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD MAR 17 PY 2015 VL 49 IS 6 BP 3383 EP 3391 DI 10.1021/es505793t PG 9 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA CD8DC UT WOS:000351324400015 PM 25700170 ER PT J AU Carlson, HK Stoeva, MK Justice, NB Sczesnak, A Mullan, MR Mosqueda, LA Kuehl, JV Deutschbauer, AM Arkin, AP Coates, JD AF Carlson, Hans K. Stoeva, Magdalena K. Justice, Nicholas B. Sczesnak, Andrew Mullan, Mark R. Mosqueda, Lorraine A. Kuehl, Jennifer V. Deutschbauer, Adam M. Arkin, Adam P. Coates, John D. TI Monofluorophosphate Is a Selective Inhibitor of Respiratory Sulfate-Reducing Microorganisms SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID DESULFOVIBRIO-VULGARIS HILDENBOROUGH; ATP SULFURYLASE; SODIUM MONOFLUOROPHOSPHATE; MARINE-SEDIMENTS; REDUCTION; BACTERIA; DESULFURICANS; FLUORIDE; SULFIDE; NITRITE AB Despite the environmental and economic cost of microbial sulfidogenesis in industrial operations, few compounds are known as selective inhibitors of respiratory sulfate reducing microorganisms (SRM), and no study has systematically and quantitatively evaluated the selectivity and potency of SRM inhibitors. Using general, high-throughput assays to quantitatively evaluate inhibitor potency and selectivity in a model sulfate-reducing microbial ecosystem as well as inhibitor specificity for the sulfate reduction pathway in a model SRM, we screened a panel of inorganic oxyanions. We identified several SRM selective inhibitors including selenate, selenite, tellurate, tellurite, nitrate, nitrite, perchlorate, chlorate, monofluorophosphate, vanadate, molydate, and tungstate. Monofluorophosphate (MFP) was not known previously as a selective SRM inhibitor, but has promising characteristics including low toxicity to eukaryotic organisms, high stability at circumneutral pH, utility as an abiotic corrosion inhibitor, and low cost. MFP remains a potent inhibitor of SRM growing by fermentation, and MFP is tolerated by nitrate and perchlorate reducing microorganisms. For SRM inhibition, MFP is synergistic with nitrite and chlorite, and could enhance the efficacy of nitrate or perchlorate treatments. Finally, MFP inhibition is multifaceted. Both inhibition of the central sulfate reduction pathway and release of cytoplasmic fluoride ion are implicated in the mechanism of MFP toxicity. C1 [Carlson, Hans K.; Mullan, Mark R.; Mosqueda, Lorraine A.; Coates, John D.] Univ Calif Berkeley, Energy Biosci Inst, Berkeley, CA 94720 USA. [Justice, Nicholas B.; Kuehl, Jennifer V.; Deutschbauer, Adam M.; Arkin, Adam P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Coates, John D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Stoeva, Magdalena K.; Coates, John D.] Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. [Sczesnak, Andrew; Arkin, Adam P.] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. RP Coates, JD (reprint author), Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. EM jdcoates@berkeley.edu RI Arkin, Adam/A-6751-2008; OI Arkin, Adam/0000-0002-4999-2931; Sczesnak, Andrew/0000-0002-0152-9745 FU Energy Biosciences Institute FX We thank members of the Coates and Arkin groups for critical comments on this manuscript. Work in the laboratory of J.D.C. on biosouring is supported by the Energy Biosciences Institute. NR 56 TC 5 Z9 5 U1 3 U2 27 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD MAR 17 PY 2015 VL 49 IS 6 BP 3727 EP 3736 DI 10.1021/es505843z PG 10 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA CD8DC UT WOS:000351324400055 PM 25698072 ER PT J AU Triantafyllidou, S Schock, MR DeSantis, MK White, C AF Triantafyllidou, Simoni Schock, Michael R. DeSantis, Michael K. White, Colin TI Low Contribution of PbO2-Coated Lead Service Lines to Water Lead Contamination at the Tap SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID CORROSION PRODUCT PBO2; DRINKING-WATER; PIPE SCALES; DISSOLUTION; FLOW; DIFFUSION; EXPOSURE; SYSTEMS; RATES AB To determine if residential water sampling corroborates the expectation that formation of stable PbO2 coatings on lead servke lines (LSLs) provides an effective lead release control strategy, lead profile sampling was evaluated for eight home kitchen taps in three US. cities with observed PbO2-coated LSLs (Newport, Rhode Island; Cincinnati and Oakwood, Ohio). After various water standing times, these LSLs typically released similar or,lower peak lead levels (1 to 18 mu g/L) than the lead levels from the respective kitchen faucets (1 to 130 mu g/L); and frequently 50-80% lower than the lead levels typically reported from Pb(II)-coated LSLs in comparable published sampling studies. Prolonged stagnation (10-101 h) at the Cincinnati sites produced varying results. One site showed minimal (0-4 mu g/L) increase in lead release from the PbO2-coated LSL, and persistence of free chlorine residual. However, the other site showed up to a 3-fold increase proportional to standing time) with essentially full depletion of the chlorine residual. Overall, lead release was consistently much lower than that reported in studies of Pb(II)-coated LSL scales, suggesting that natural formation of PbO2 in LSLs is an effective lead "corrosion" control strategy. C1 [Triantafyllidou, Simoni; DeSantis, Michael K.] US EPA, ORISE, Cincinnati, OH 45268 USA. [Schock, Michael R.] US EPA, Water Supply & Water Resources Div, Natl Risk Management Res Lab, Cincinnati, OH 45268 USA. [White, Colin] Univ Cincinnati, Dept Biomed Chem & Environm Engn, Coll Engn & Appl Sci, Cincinnati, OH 45221 USA. RP Schock, MR (reprint author), US EPA, Water Supply & Water Resources Div, Natl Risk Management Res Lab, Cincinnati, OH 45268 USA. EM schock.michael@epa.gov FU US DOE Office of Science [DEFG03-97ER45628]; U.S. DOE, Office of Science, Office of Basic Energy Sciences [W-31-109-Eng-38] FX We thank Dr. John Eastman (LJB Engineers, Inc.), and Barbara Wysock (formerly USEPA Office of Drinking Water) for the Oakwood study, as well as Carol Rego and Kathy Mello (CDM) for the Newport study. Norb Klopsch (City of Oakwood), Jeff Swertfeger and Dawn Webb (Greater Cincinnati Water Works) provided pipe specimens. Keith Kelty, Maily Pham, and Bill Kaylor (USEPA Office of Research and Development) conducted water metals analyses. All pipe scale elemental analyses were conducted by the USGS Mineral Resource Surveys Program under the direction of Dr. Stephen A. Wilson. All XANES analyses were supported by the US DOE Office of Science Grant No. DEFG03-97ER45628 and were conducted in the PNC-CAT facilities at the Advanced Photon Source, Argonne National Laboratory, Argonne, IL. A.P.S. is supported by the U.S. DOE, Office of Science, Office of Basic Energy Sciences, under Contract No. W-31-109-Eng-38. This project was supported in part by an appointment to the Research Participation Program at the Office of research and Development, USEPA, administered by the Oak Ridge Institute for Science and Education through an interagency agreement between the U.S. Department of Energy and USEPA. Any opinions expressed in this paper are those of the authors and do not necessarily reflect the official position and policies of the USEPA. NR 49 TC 3 Z9 3 U1 5 U2 23 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD MAR 17 PY 2015 VL 49 IS 6 BP 3746 EP 3754 DI 10.1021/es505886h PG 9 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA CD8DC UT WOS:000351324400057 PM 25692317 ER PT J AU Salter-Blanc, AJ Bylaska, EJ Johnston, HJ Tratnyek, PG AF Salter-Blanc, Alexandra J. Bylaska, Eric J. Johnston, Hayley J. Tratnyek, Paul G. TI Predicting Reduction Rates of Energetic Nitroaromatic Compounds Using Calculated One-Electron Reduction Potentials SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID NITROGEN ISOTOPE FRACTIONATION; DENSITY-FUNCTIONAL METHODS; ABIOTIC REDUCTION; AQUEOUS-MEDIUM; RATE CONSTANTS; BASIS-SET; CONTAMINANTS; KINETICS; IRON(II); THERMOCHEMISTRY AB The evaluation of new energetic nitroaromatic compounds (NACs) for use in green munitions formulations requires models that can predict their environmental f4te. Previously invoked linear free energy relationships (LFER) relating the log of the rate constant for this reaction (log(k)) and one-electron reduction potentials for the NAC (E-NAC(1)) normalized to 0.059 V have been re-evaluated and compared to a new analysis using a (nonlinear) free-energy relationship (FER) based On the Marcus theory of outersphere electron transfer. For most reductants, the results are inconsistent with simple rate limitation by an initial, outer-sphere electron transfer, suggesting that the linear correlation between log(k) and E-NAC(1) is best regarded as an empirical model. This correlation was used to calibrate a new quantitative structure-activity relationship (QSAR) using previously reported values of log(k) for nonehergetic NAC reduction by Fe(II) porphyrin and newly reported values of E-NAC(1) determined using density functional theory at the M06-2X/6-311++G(2d,2p) level with the COSMO solvation model. The QSAR was then validated for energetic NACs using newly measured kinetic data for 2,4,6-trinitrotoluehe (TNT), 2,4-dinitrotoluene (2,4-DNT), and 2,4-dinitroanisole (DNAN). The data show close agreement with the QSAR, supporting its applicability to other energetic NACs. C1 [Salter-Blanc, Alexandra J.; Johnston, Hayley J.; Tratnyek, Paul G.] Oregon Hlth & Sci Univ, Inst Environm Hlth, Portland, OR 97239 USA. [Bylaska, Eric J.] Pacific NW Natl Lab, William R Wiley Environm Mol Sci Lab, Richland, WA 99352 USA. RP Tratnyek, PG (reprint author), Oregon Hlth & Sci Univ, Inst Environm Hlth, 3181 SW Sam Jackson Pk Rd, Portland, OR 97239 USA. EM tratnyek@ohsu.edu FU Strategic Environmental Research and Development Program (SERDP) [ER-1735]; OHSU; Department of Energy's Office of Biological and Environmental Research located at Pacific Northwest National Laboratory [DE-AC06-76RLO 1830]; EMSL FX This work was supported by the Strategic Environmental Research and Development Program (SERDP) under ER-1735. This report has not been subject to review by SERDP and therefore does not necessarily reflect their views and no official endorsement should be inferred. A. J. S.-B. was supported as an OHSU Graduate Research Scholar during a portion of this study. A portion of this research was performed using the PNNL Institutional Computing (PIC) facility and the Chinook, Spokane, Barracuda, and Cascade computing resources at the Molecular Science Computing Facility at EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research located at Pacific Northwest National Laboratory, DE-AC06-76RLO 1830. We also acknowledge EMSL for supporting the development of NWChem. The Pacific Northwest National Laboratory is operated by Battelle Memorial Institute. Structure database management and sorting was performed using Instant JChem (Instant JChem 5.9.4, 2012, Chem Axon (http://www.chemaxon.com)). NR 52 TC 3 Z9 3 U1 11 U2 55 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD MAR 17 PY 2015 VL 49 IS 6 BP 3778 EP 3786 DI 10.1021/es505092s PG 9 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA CD8DC UT WOS:000351324400061 PM 25671710 ER PT J AU McGee, MA Kamal, AS McGee, JK Wood, CE Dye, JA Krantz, QT Landis, MS Gilmour, MI Gavett, SH AF McGee, Marie A. Kamal, Ali S. McGee, John K. Wood, Charles E. Dye, Janice A. Krantz, Q. Todd Landis, Matthew S. Gilmour, M. Ian Gavett, Stephen H. TI Differential Effects of Particulate Matter Upwind and Downwind of an Urban Freeway in an Allergic Mouse Model SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID OIL FLY-ASH; AIR-POLLUTION PARTICLES; NEAR-ROAD EXPOSURES; SOURCE APPORTIONMENT; CHEMICAL-COMPOSITION; RESPIRATORY HEALTH; UNITED-STATES; LUNG-FUNCTION; IN-VITRO; COARSE AB Near-road exposure to air pollutants has been associated with decreased lung function and other adverse health effects in susceptible populations. This study was designed to investigate whether different types of near,road particulate matter (PM) contribute to exacerbation of allergic asthma. Samples of upwind and downwind coarse, fine, and ultrafine PM were collected using a wind direction-actuated ChemVol sampler at a single site 100 in from Interstate-96 in Detroit, MI during winter 2010/2011. Upwind PM was enriched in crustal and wood combustion sources while downwind PM was dominated by traffic sources. Control and ovalbumin (OVA)-sensitized BALB/cJ Mice were exposed Via oropharyngeal (OP) aspiration to 20 or 100 mu g of each PM sample 2 h prior to OP challenge with OVA. In OVA-allergic mice, 100 mu g Of downwind coarse PM caused greater increase than downwind fine/ultrafine PM in bronchoalveolar lavage neutrophils, eosinophils, and lactate dehydrogenase. Upwind fine PM (100 mu g) produced greater increases in heutrophils and eosinophils compared to other upwind size fractions. Cytokine (IL-5) levels in BAL fluid also increased markedly following 100 mu g downwind coarse and downwind ultrafine PM exposures. These findings indicate coarse PM downwind and line PM upwind of an interstate highway promote inflammation in allergic mice. C1 [McGee, Marie A.] Univ N Carolina, Curriculum Toxicol, Chapel Hill, NC 27599 USA. [Kamal, Ali S.] Oak Ridge Inst Sci & Educ, Res Triangle Pk, NC 27711 USA. [McGee, John K.; Wood, Charles E.; Dye, Janice A.; Krantz, Q. Todd; Landis, Matthew S.; Gilmour, M. Ian; Gavett, Stephen H.] US EPA, Natl Hlth & Environm Effects Res Lab, Off Res & Dev, Res Triangle Pk, NC 27711 USA. RP Gavett, SH (reprint author), US EPA, Mail Code B105-02, Res Triangle Pk, NC 27711 USA. EM gavett.stephen@epa.gov OI McGee, Marie/0000-0001-8572-1613 FU EPA-UNC training agreement, Curriculum in Toxicology, University of North Carolina at Chapel Hill [CR83515201-0] FX The authors thank Debora Andrews, Elizabeth Boykin, Lisa Copeland, Mary Daniels, Eugene Gibbs, Richard Jaskot, Kasey Kovalcik, Jim Lehmann, and Judy Richards for technical assistance, and Drs. Janet Burke and Marsha Ward for paper review. This project was supported by the EPA-UNC training agreement, Curriculum in Toxicology, University of North Carolina at Chapel Hill (CR83515201-0). NR 52 TC 4 Z9 4 U1 2 U2 11 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD MAR 17 PY 2015 VL 49 IS 6 BP 3930 EP 3939 DI 10.1021/es506048k PG 10 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA CD8DC UT WOS:000351324400078 PM 25710269 ER PT J AU Mitchell, JM Clasman, JR June, CM Kaitany, KCJ LaFleur, JR Taracila, MA Klinger, NV Bonomo, RA Wymore, T Szarecka, A Powers, RA Leonard, DA AF Mitchell, Joshua M. Clasman, Jozlyn R. June, Cynthia M. Kaitany, Kip-Chumba J. LaFleur, James R. Taracila, Magdalena A. Klinger, Neil V. Bonomo, Robert A. Wymore, Troy Szarecka, Agnieszka Powers, Rachel A. Leonard, David A. TI Structural Basis of Activity against Aztreonam and Extended Spectrum Cephalosporins for Two Carbapenem-Hydrolyzing Class D beta-Lactamases from Acinetobacter baumannii SO BIOCHEMISTRY LA English DT Article ID CRYSTAL-STRUCTURE; PSEUDOMONAS-AERUGINOSA; MOLECULAR-DYNAMICS; CLASS-A; CEFTAZIDIME; RESISTANCE; INHIBITOR; MECHANISM; COMPLEX; PROTEIN AB The carbapenem-hydrolyzing class D beta-lactamases OXA-23 and OXA-24/40 have emerged worldwide as causative agents for beta-lactam antibiotic resistance in Acinetobacter species. Many Variants of these enzymes have appeared clinically, including OXA-160 and OXA-225, which both contain a P -> S substitution at homologous positions in the OXA-24/40 and OXA-23 background's, respectively. We purified OXA-160 and OXA-225 and used steady-State kinetic analysis to compare the substrate profiles of these variants to their parental enzymes, OXA-24/40 and OXA-23. OXA-160 and OXA-225 possess greatly enhanced hydrolytic activities against aztreonam, ceftazidime, cefotaxime, and ceftriaxone when compared to OXA-24/40 and OXA-23. These enhanced activities are the result of much lower K-m values, suggesting that the P -> S substitution enhances the binding affinity of these drugs. We have determined the structures of the acylated forms of OXA-160 (with ceftazidime and aztreonam) and OXA-225 (ceftazidime). These structures show that the R1 oxyimino side-chain of these drugs occupies a space near the beta 5-beta 6 loop and the omega loop of the enzymes. The P -> S substitution found in OXA-160 and OXA-225 results in a deviation of the beta 5-beta 6 loop, relieving the steric dash with the R1 side-chain carboxypropyl group of aztreonam and ceftazidime. These results reveal worrying trends in the enhancement of substrate spectrum of class beta-lactamases but may also provide a map for Chi-lactam improvement. C1 [Mitchell, Joshua M.; Clasman, Jozlyn R.; June, Cynthia M.; Kaitany, Kip-Chumba J.; Klinger, Neil V.; Powers, Rachel A.; Leonard, David A.] Grand Valley State Univ, Dept Chem, Allendale, MI 49401 USA. [LaFleur, James R.; Szarecka, Agnieszka] Grand Valley State Univ, Dept Cell & Mol Biol, Allendale, MI 49401 USA. [Taracila, Magdalena A.; Bonomo, Robert A.] Case Western Reserve Univ, Dept Med, Cleveland, OH 44106 USA. [Taracila, Magdalena A.; Bonomo, Robert A.] Case Western Reserve Univ, Dept Pharmacol, Cleveland, OH 44106 USA. [Taracila, Magdalena A.; Bonomo, Robert A.] Case Western Reserve Univ, Dept Biochem, Cleveland, OH 44106 USA. [Taracila, Magdalena A.; Bonomo, Robert A.] Case Western Reserve Univ, Dept Mol Biol & Microbiol, Cleveland, OH 44106 USA. [Taracila, Magdalena A.; Bonomo, Robert A.] Res Serv, Cleveland, OH 44106 USA. [Taracila, Magdalena A.; Bonomo, Robert A.] Louis Stokes Cleveland Dept Vet Affairs Med Ctr, Cleveland, OH 44106 USA. [Wymore, Troy] Oak Ridge Natl Lab, UT ORNL Ctr Mol Biophys, Biosci Div, Oak Ridge, TN 37831 USA. RP Leonard, DA (reprint author), Grand Valley State Univ, Dept Chem, Allendale, MI 49401 USA. EM leonardd@gvsu.edu FU National Institutes of Health [1R15AI082416, R15AI094489]; Cleveland Department of Veterans Affairs; Department of Veterans Affairs Merit Review Program [1I01BX001974]; Veterans Integrated Service Network 10 Geriatric Research, Education, and Clinical Center (VISN 10 GRECC); National Institute of Allergy and Infectious Diseases of the National Institutes of Health [R01 AI100560, R01 AI063517]; National Center for Multiscale Modeling of Biological Systems (MMBioS) through National Institutes of Health [P41GM103712]; U.S. DOE [DE-AC02-06CH11357]; Michigan Economic Development Corporation; Michigan Technology Tri-Corridor [085P1000817] FX This research was supported by National Institutes of Health Grant 1R15AI082416 (D.A.L.) and R15AI094489 (R.A.P). Additional support was also provided by the Cleveland Department of Veterans Affairs, the Department of Veterans Affairs Merit Review Program 1I01BX001974, the Veterans Integrated Service Network 10 Geriatric Research, Education, and Clinical Center (VISN 10 GRECC), and the National Institute of Allergy and Infectious Diseases of the National Institutes of Health under Award Numbers R01 AI100560 and R01 AI063517 (R.A.B). This work was also supported by the National Center for Multiscale Modeling of Biological Systems (MMBioS) through National Institutes of Health Grant P41GM103712 (T.W.). Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. Use of the LS-CAT Sector 21 was supported by the Michigan Economic Development Corporation and the Michigan Technology Tri-Corridor (Grant 085P1000817). NR 55 TC 6 Z9 6 U1 1 U2 5 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0006-2960 J9 BIOCHEMISTRY-US JI Biochemistry PD MAR 17 PY 2015 VL 54 IS 10 BP 1976 EP 1987 DI 10.1021/bi501547k PG 12 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CD8EU UT WOS:000351328800012 PM 25710192 ER PT J AU Aad, G Abbott, B Abdallah, J Khalek, SA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Agatonovic-Jovin, T Aguilar-Saavedra, JA Agustoni, M Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TPA Akimoto, G Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Allbrooke, BMM Allison, LJ Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Coutinho, YA Amelung, 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TI Search for charged Higgs bosons decaying via H-+/- -> tau(+/-)nu in fully hadronic final states using pp collision data at root s=8 TeV with the ATLAS detector SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Supersymmetry; Hadron-Hadron Scattering; Beyond Standard Model; Higgs physics ID NEUTRINO MASSES; MONTE-CARLO; MSSM; SUPERSYMMETRY; PHENOMENOLOGY; VIOLATION; MIXINGS; MODELS; WEAK AB The results of a search for charged Higgs bosons decaying to a T lepton and a neutrino. H-+/- -> T-+/-nu, are presented. The analysis is based on 19.5 fb(-1) of proton-proton collision data at root s = 8 TeV collected by the ATLAS experiment at the Large Hadron Collider. Charged Higgs bosons are searched for in events consistent with top-quark pair production or in associated production with a top quark, depending on the considered H-+/- mass. The final state is characterised by the presence of a hadronic T decay, missing transverse momentum, b-tagged jets, a hadronically decaying W boson, and the absence of any isolated electrons or unions with high transverse momenta. The data are consistent with the expected background from Standard Model processes. A statistical analysis leads to 95% confidence-level upper limits on the product of branching ratios B(t -> bH(+/-)) x B(H-+/- -> T-+/-nu), between 0.23% and 1.3% for charged Higgs boson masses in the range 80 160 GeV. lit also leads to 95% confidence-level upper limits on the production cross section times branching ratio, sigma(pp -> tH(+/-) + X) x B(H-+/--> T(+/-)v), between 0.76 pb and 4.5 fb, for charged Higgs boson masses ranging from 180 GeV to 1000 GeV. In the context of different scenarios of the Minimal Supersymnietric Standard Model, these results exclude nearly all values of tan beta above one for charged Higgs boson masses between 80 GeV and 160 GeV, and exclude a region of parameter space with high tan beta for H-+/- masses between 200 GeV and 250 GeV. C1 [Jackson, P.; Lee, L.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Edson, W.; Ernst, J.; Fischer, A.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Butt, A. I.; Czodrowski, P.; Gingrich, D. M.; Karamaoun, A.; Moore, R. W.; Pinfold, J. L.; Saddique, A.; Vaque, F. Vives] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakir, O.; Ciftci, A. K.; Ciftci, R.; Yildiz, H. Duran] Ankara Univ, Dept Phys, TR-06100 Ankara, Turkey. [Yilmaz, M.] Gazi Univ, Dept Phys, Ankara, Turkey. [Kuday, S.; Cakir, I. Turk] Istanbul Aydin Univ, Istanbul, Turkey. [Sultansoy, S.] TOBB Univ Econ & Technol, Div Phys, Ankara, Turkey. 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L.; Caforio, D.; De Castro, S.; Di Sipio, R.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Grafstroem, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Piccinini, M.; Romano, M.; Sbrizzi, A.; Semprini-Cesari, N.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, Dipartimento Fis & Astron, Bologna, Italy. [Arslan, O.; Bechtle, P.; Bernlochner, F. U.; Brock, I.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Ehrenfeld, W.; Gaycken, G.; Geich-Gimbel, Ch.; Gonella, L.; Haefner, P.; Hageboeck, S.; Hellmich, D.; Huegging, F.; Janssen, J.; Khoriauli, G.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lapoire, C.; Lenz, T.; Leyko, A. M.; Liebal, J.; Limbach, C.; Mergelmeyer, S.; Mijovic, L.; Miller, D. W.; Mueller, K.; Nanava, G.; Nattermann, T.; Obermann, T.; Pohl, D.; Sarrazin, B.; Schaepe, S.; Schultens, M. J.; Schwindt, T.; Scutti, F.; Seema, P.; Stillings, J. A.; Tannoury, N.; Therhaag, J.; Uhlenbrock, M.; Velz, T.; Vogel, A.; von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Winter, B. T.; Wong, K. H. Yau; Zimmermann, R.; Zimmermann, S.] Univ Bonn, Inst Phys, Bonn, Germany. [Ahlen, S. P.; Bernard, C.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Long, B. A.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Inst Phys, Boston, MA 02215 USA. [Amelung, C.; Amundsen, G.; Artoni, G.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Fitzgerald, E. A.; Sciolla, G.; Venturini, A.; Zambito, S.; Zengel, K.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Coutinho, Y. Amaral; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio de Janeiro, COPPE, EE, IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; de Andrade Filho, L. Manhaes] Fed Univ Juiz de Fora UFJF, Elect Circuits Dept, Juiz De Fora, Brazil. [do Vale, M. A. B.] Fed Univ Sao Joao del Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadelli, M.; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Boscherini, D.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Kaneti, S.; Klimentov, A.; Kouskoura, V.; Kravchenko, A.; Lanni, F.; Lester, C. G.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Metcalfe, J.; Mountricha, E.; Nevski, P.; Nilsson, P.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Perepelitsa, D. V.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Schovancova, J.; Snyder, S.; Steinberg, P.; Takai, H.; Undrus, A.; Wenaus, T.; Ye, S.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Badescu, E.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Dita, P.; Dita, S.; Ducu, O. A.; Jinaru, A.; Maurer, J.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Otero y Garzon, G.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Buttinger, W.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Gillam, T. P. S.; Hill, J. C.; Khoo, T. J.; Mueller, T.; Parker, M. A.; Robinson, D.; Sandoval, T.; Thomson, M.; Ward, C. P.; Williams, S.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Leight, W. A.; Marchand, J. F.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Abreu, R.; Aleksa, M.; Andari, N.; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Battistin, M.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Conti, G.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duehrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Perez, S. Fernandez; Franchino, S.; Francis, D.; Froidevaux, D.; Garonne, V.; Gianotti, F.; Gillberg, D.; Glatzer, J.; Godlewski, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hauschild, M.; Hawkings, R. J.; Heller, M.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Hubacek, Z.; Huhtinen, M.; Jaekel, M. R.; Jakobsen, S.; Jansen, H.; Kaneda, M.; Klioutchnikova, T.; Krasznahorkay, A.; Lantzsch, K.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Martin, B.; Marzin, A.; Messina, A.; Meyer, J.; Milic, A.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Negri, G.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Pommes, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Rodrigues, L.; Roe, S.; Ruiz-Martinez, A.; Salzburger, A.; Savu, D. O.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van der Ster, D.; van Eldik, N.; van Woerden, M. C.; Vandelli, W.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Anderson, K. J.; Boveia, A.; Cheng, Y.; Facini, G.; Fiascaris, M.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Krizka, K.; Li, H. L.; Meehan, S.; Melachrinos, C.; Merritt, F. S.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Tompkins, L.; Vukotic, I.; Webster, J. S.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carquin, E.; Diaz, M. A.; Vogel, M.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lou, X.; Lu, F.; Ouyang, Q.; Ren, H.; Shan, L. Y.; Sun, X.; Wang, J.; Xu, D.; Yao, L.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guan, L.; Han, L.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, K.; Liu, M.; Liu, Y.; Peng, H.; Song, H. Y.; Xu, L.; Zhang, R.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Wang, C.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200030, Peoples R China. [Chen, X.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Podlyski, F.; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Clermont Univ, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Podlyski, F.; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Podlyski, F.; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] CNRS, IN2P3, Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Cole, B.; Guo, J.; Hu, D.; Hughes, E. W.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, INFN, Grp Collegato Cosenza, Lab Nazl Frascati, Arcavacata Di Rende, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Palka, M.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. 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S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Medinnis, M.; Moenig, K.; Morton, A.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Hamburg, Germany. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Borroni, S.; Camarda, S.; Deterre, C.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Belenguer, M. Jimenez; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Medinnis, M.; Moenig, K.; Morton, A.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Erdmann, J.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Kobel, M.; Mader, W. F.; Morgenstern, M.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Edwards, N. C.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, Sch Phys & Astron, SUPA, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Buescher, D.; Coniavitis, E.; Consorti, V.; Dao, V.; Di Simone, A.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Madar, R.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Rave, T. C.; Ronzani, M.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; von Radziewski, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Alexandre, G.; Ancu, L. S.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Bucci, F.; Toro, R. Camacho; Clark, A.; Delitzsch, C. M.; della Volpe, D.; Dias, F. A.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Goulette, M. P.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Nektarijevic, S.; Nessi, M.; Nikolics, K.; Picazio, A.; Pohl, M.; Rosbach, K.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Univ Genoa, Ist Nazl Fis Nucl, Sez Genova, Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, GE-380086 Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Phys Inst 2, D-35390 Giessen, Germany. [Bates, R. L.; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; Mullen, P.; O'Shea, V.; Barrera, C. Oropeza; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; Saxon, D. H.; Smith, K. M.; Denis, R. D. St.; Stewart, G. A.; Thompson, A. S.; Wright, M.] Univ Glasgow, Sch Phys & Astron, SUPA, Glasgow, Lanark, Scotland. [Bierwagen, K.; Bindi, M.; Blumenschein, U.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Kareem, M. J.; Kawamura, G.; Keil, M.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Stolte, P.; Schroeder, T. Vazquez; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Phys Inst 2, D-37073 Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS, IN2P3, Lab Phys Subat & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Butler, B.; Catastini, P.; Franklin, M.; Huth, J.; Ippolito, V.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Yen, A. L.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Dietzsch, T. A.; Djuvsland, J. I.; Dunford, M.; Hanke, P.; Jongmanns, J.; Khomich, A.; Kluge, E. -E.; Laier, H.; Lang, V. S.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Heidelberg, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Castillo, L. R. Flores] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Brunet, S.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Glonti, G. L.; Jussel, P.; Kneringer, E.; Lukas, W.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Mallik, U.; Mandrysch, R.; Morange, N.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Pluth, D.; Prell, S.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Kazarinov, M. Y.; Khramov, E.; Kruchonak, U.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Topilin, N. D.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] KEK, High Energy Accelerator Res Org, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Inamaru, Y.; Kishimoto, T.; Kurashige, H.; Kurumida, R.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Verzini, M. J. Alconada; Alonso, F.; Anduaga, X. S.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Verzini, M. J. Alconada; Alonso, F.; Anduaga, X. S.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Allison, L. J.; Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Orlando, N.; Primavera, M.; Spagnolo, S.; Ventura, A.] Univ Salento, Ist Nazl Fis Nucl, Sez Lecce, Lecce, Italy. [Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dassoulas, J.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Readioff, N. P.; Schnellbach, Y. J.; Sellers, G.; Vossebeld, J. H.; Waller, P.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bevan, A. J.; Bona, M.; Bret, M. Cano; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cooper-Smith, N. J.; Cowan, G.; Duguid, L.; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Rose, M.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Cooper, B. D.; Davison, A. R.; Davison, P.; Falla, R. J.; Gregersen, K.; Gutschow, C.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, I.; Pilkington, A. D.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Jana, D. K.; Sawyer, L.; Sircar, A.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjoernmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Inst Fys, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lin, T. H.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Poettgen, R.; Rave, S.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, D-55122 Mainz, Germany. [Barnes, S. L.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Peters, R. F. Y.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Robinson, J. E. M.; Schwanenberger, C.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Clemens, J. C.; Coadou, Y.; Diglio, S.; Djama, F.; Feligioni, L.; Hallewell, G. D.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Liu, J.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Clemens, J. C.; Coadou, Y.; Diglio, S.; Djama, F.; Feligioni, L.; Hallewell, G. D.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Liu, J.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Jennens, D.; Kubota, T.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Dubbert, J.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Hu, X.; Levin, D.; Liu, L.; Long, J. D.; Lu, N.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Panikashvili, N.; Qian, J.; Schwarz, T. A.; Searcy, J.; Thun, R. P.; Wilson, A.; Wu, Y.; Xu, L.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Koll, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Citterio, M.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazza, S. M.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Univ Milan, Ist Nazl Fis Nucl, Sez Milano, Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Mazza, S. M.; Perini, L.; Pizio, C.; Ragusa, F.; Shojaii, S.; Simoniello, R.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus. [Hrynevich, A.; Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] ITEP, Moscow, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Chelkov, G. A.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Tikhomirov, V. 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A.; Manfredini, A.; Menke, S.; Moser, H. G.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Pahl, C.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Spettel, F.; Stern, S.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Chiefari, G.; Conventi, F.; De Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Patricelli, S.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Univ Naples Federico II, Ist Nazl Fis Nucl, Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Chiefari, G.; Di Donato, C.; Giordano, R.; Merola, L.; Patricelli, S.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Klok, P. F.; Koenig, A. C.; Salvucci, A.; Strubig, A.] Radboud Univ Nijmegen Nikhel, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Oussoren, K. P.; Pani, P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Adelman, J.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL USA. [Anisenkov, A. V.; Bogdanchikov, A. G.; Kazanin, V. F.; Kharlamov, A.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Badker Inst Nucl Phys, Novosibirsk, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, New York, NY 10003 USA. [Beacham, J. B.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; Gutierrez, P.; Hasib, A.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Bousson, N.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] CNRS, IN2P3, F-91405 Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Read, A. L.; Rohne, O.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, K.; Boddy, C. R.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; King, R. S. B.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pachal, K.; Pickering, M. A.; Pinder, A.; Ryder, N. C.; Sawyer, C.; Short, D.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Univ Pavia, INFN, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Kroll, J.; Lester, C. M.; Lipeles, E.; Meyer, C.; Ospanov, R.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Vanguri, R.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Volpi, G.; White, S.] Univ Pisa, Ist Nazl Fis Nucl, Sez Pisa, I-56100 Pisa, Italy. [Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Volpi, G.; White, S.] Univ Pisa, Dipartirnento Fis E Fermi, I-56100 Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Mueller, J.; Prieur, D.; Sapp, K.; Su, J.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Dos Santos, S. P. Amor; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Miguens, J. Machado; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] LIP, Lab Instrumentac & Fis Expt Particulas, P-1000 Lisbon, Portugal. [Amorim, A.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Dos Santos, S. P. Amor; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, CETITEC, Fac Ciencias & Tecnol, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Gallus, P.; Guenther, J.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Leitner, R.; Pleskot, V.; Reznicek, P.; Rybar, M.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Aloisio, A.; Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] Inst High Energy Phys, State Res Ctr, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Tanaka, S.] Ritsumeikan Univ, Shiga, Japan. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Sidoti, A.; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Ist Nazl Fis Nucl, Sez Roma, I-00185 Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; Di Domenico, A.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Iuppa, R.; Liberti, B.; Mazzaferro, L.; Paolozzi, L.; Salamon, A.; Santonico, R.] Univ Roma Tor Vergata, Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Iuppa, R.; Mazzaferro, L.; Paolozzi, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Stanescu, C.; Taccini, C.; Trovatelli, M.] Univ Rome Tre, Ist Nazl Fis Nucl, Sez Roma Tre, I-00146 Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Taccini, C.; Trovatelli, M.] Univ Rome Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Tech, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA, Fac Sci Semlalia, Marrakech, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mal, P.; Mansoulie, B.; Martinez, H.; Meric, N.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.; Tsionou, D.; Vranjes, N.; Xiao, M.] CEA Saclay, Commissariat Energie Atom & Energies Alternat, DSM IRFU, F-91191 Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grabas, H. M. X.; Grillo, A. A.; Kuhl, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Miyagawa, P. S.; Paganis, E.; Tovey, D. R.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Dawe, E.; Horton, A. J.; O'Neil, D. C.; Stelzer, B.; Tanasijczuk, A. J.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Kagan, M.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nef, P. D.; Nelson, T. K.; Piacquadio, G.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Strauss, E.; Su, D.; Swiatlowski, M.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Federic, P.; Plazak, L.; Stavina, P.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Connell, S. H.; Lee, C. A.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Carrillo-Montoya, G. D.; Hamity, G. N.; Hsu, C.; March, L.; Garcia, B. R. Mellado; Ruan, X.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjoelin, J.; Strandberg, S.; Tylmad, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Gellerstedt, K.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Shcherbakova, A.; Sjoelin, J.; Strandberg, S.; Tylmad, M.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Asquith, L.; Bartsch, V.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Chu, M. L.; De Santo, A.; Hou, S.; Hsu, P. J.; Jamin, D. O.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Ren, Z. L.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, S. M.; Weng, Z.; Zhang, L.] Acad Sinica, Inst Phys, Taipei 115, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Guttman, N.; Munwes, Y.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Papageorgiou, K.; Hernandez, D. Paredes; Petridou, C.; Sampsonidis, D.; Sidiropoulou, O.] Aristotle Univ Thessaloniki, Dept Phys, Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Nobe, T.; Pettersson, N. E.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Brelier, B.; Chau, C. C.; DeMarco, D. A.; Ilic, N.; Keung, J.; Krieger, P.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Schramm, S.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Gingrich, D. M.; Koutsman, A.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.; Qureshi, A.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Moreno, D.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Rao, K.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Quayle, W. B.; Shaw, K.; Soualah, R.] Ist Nazl Fis Nucl, Grp Colegato Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; Quayle, W. B.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Errede, S.; Lie, K.; Liss, T. M.; Neubauer, M. S.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Kuutmann, E. Bergeaas; Brenner, R.; Buszello, C. P.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] CSIC, Valencia, Spain. [Danninger, M.; Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC V5Z 1M9, Canada. [Albert, J.; Berghaus, F.; David, C.; Elliot, A. A.; Fincke-Keeler, M.; Hamano, K.; Hill, E.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Marino, C. P.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.; Venturi, M.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Beckingham, M.; Farrington, S. M.; Harrison, P. F.; Janus, M.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Barak, L.; Bressler, S.; Citron, Z. H.; Duchovni, E.; Gross, E.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Pitt, M.; Roth, I.; Schaarschmidt, J.; Smakhtin, V.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Heng, Y.; Ji, H.; Ju, X.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Kuger, F.; Redelbach, A.; Schreyer, M.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Univ Wurzburg, Fac Phys & Astron, D-97070 Wurzburg, Germany. [Bannoura, A. A. E.; Barisonzi, M.; Beermann, T. A.; Boek, T. T.; Braun, H. M.; Cornelissen, T.; Duda, D.; Ernis, G.; Fischer, J.; Fleischmann, S.; Flick, T.; Gabizon, O.; Hamacher, K.; Hard, A. S.; Harenberg, T.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Kohlmann, S.; Lenzen, G.; Maettig, P.; Neumann, M.; Pataraia, S.; Sandhoff, M.; Sartisohn, G.; Tepel, F.; Wagner, W.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich C Phys, Wuppertal, Germany. [Baker, O. K.; Bedikian, S.; Cummings, J.; Demers, S.; Garberson, F.; Guest, D.; Henrichs, A.; Ideal, E.; Lagouri, T.; Leister, A. G.; Loginov, A.; Tipton, P.; Wall, R.; Walsh, B.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] IN2P3, Ctr Calcul, Villeurbanne, France. [Acharya, B. S.] Kings Coll London, Dept Phys, London, England. [Anisenkov, A. V.; Bobrovnikov, V. S.; Korol, A. A.; Maslennikov, A. L.; Maximov, D. A.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Bawa, H. S.; Gao, Y. S.; Lowe, A. J.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beck, H. P.] Univ Fribourg, Dept Phys, CH-1700 Fribourg, Switzerland. [Chelkov, G. A.] Tomsk State Univ, Tomsk 634050, Russia. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Corriveau, F.; McPherson, R. A.; Robertson, S. H.; Sobie, R.; Teuscher, R. J.] IPP, Toronto, ON, Canada. [Fedin, O. L.] St Petersburg State Univ, Dept Phys, St Petersburg 199034, Russia. [Grinstein, S.; Rozas, A. Juste; Martinez, M.] ICREA, Barcelona, Spain. [Hsu, P. J.] Natl Tsing Hua Univ, Dept Phys, Hsinchu, Taiwan. [Ilchenko, Y.; Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Jejelava, J.] Ilia State Univ, Inst Theoret Phys, Tbilisi, Rep of Georgia. [Jenni, P.] CERN, Geneva, Switzerland. [Kono, T.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo 112, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei 115, Taiwan. [Mal, P.] Inst Natl Sci Educ & Res, Sch Phys Sci, Bhubaneswar, Orissa, India. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Shi, L.; Soh, D. A.; Weng, Z.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Vickey, T.] Univ Oxford, Dept Phys, Oxford, England. [Wildt, M. A.] Univ Hamburg, Inst Phys Expt, Hamburg, Germany. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur 59100, Malaysia. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France. RI Ciubancan, Liviu Mihai/L-2412-2015; Zhukov, Konstantin/M-6027-2015; Shmeleva, Alevtina/M-6199-2015; Gavrilenko, Igor/M-8260-2015; Tikhomirov, Vladimir/M-6194-2015; Chekulaev, Sergey/O-1145-2015; Warburton, Andreas/N-8028-2013; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; De, Kaushik/N-1953-2013; Carvalho, Joao/M-4060-2013; Riu, Imma/L-7385-2014; Costa, Maria Jose/H-5962-2015; Cavalli-Sforza, Matteo/H-7102-2015; Marti-Garcia, Salvador/F-3085-2011; Della Pietra, Massimo/J-5008-2012; Petrucci, Fabrizio/G-8348-2012; Negrini, Matteo/C-8906-2014; Ferrer, Antonio/H-2942-2015; Grancagnolo, Sergio/J-3957-2015; Doyle, Anthony/C-5889-2009; spagnolo, stefania/A-6359-2012; Tassi, Enrico/K-3958-2015; Ferrando, James/A-9192-2012; Joergensen, Morten/E-6847-2015; Boyko, Igor/J-3659-2013; Mitsou, Vasiliki/D-1967-2009; Carquin, Edson/G-5221-2015; Mir, Lluisa-Maria/G-7212-2015; Livan, Michele/D-7531-2012; Brooks, William/C-8636-2013; Villa, Mauro/C-9883-2009; White, Ryan/E-2979-2015; Di Domenico, Antonio/G-6301-2011; Connell, Simon/F-2962-2015; Bosman, Martine/J-9917-2014; Gerbaudo, Davide/J-4536-2012; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Peleganchuk, Sergey/J-6722-2014; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Ventura, Andrea/A-9544-2015; Kantserov, Vadim/M-9761-2015; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; KHODINOV, ALEKSANDR/D-6269-2015; Staroba, Pavel/G-8850-2014; Goncalo, Ricardo/M-3153-2016; Gauzzi, Paolo/D-2615-2009; Mindur, Bartosz/A-2253-2017; Gutierrez, Phillip/C-1161-2011; Fabbri, Laura/H-3442-2012; Mashinistov, Ruslan/M-8356-2015; Buttar, Craig/D-3706-2011; Smirnova, Oxana/A-4401-2013; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Olshevskiy, Alexander/I-1580-2016; Snesarev, Andrey/H-5090-2013 OI Ciubancan, Liviu Mihai/0000-0003-1837-2841; Tikhomirov, Vladimir/0000-0002-9634-0581; Warburton, Andreas/0000-0002-2298-7315; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; De, Kaushik/0000-0002-5647-4489; Carvalho, Joao/0000-0002-3015-7821; Riu, Imma/0000-0002-3742-4582; Della Pietra, Massimo/0000-0003-4446-3368; Petrucci, Fabrizio/0000-0002-5278-2206; Negrini, Matteo/0000-0003-0101-6963; Ferrer, Antonio/0000-0003-0532-711X; Grancagnolo, Sergio/0000-0001-8490-8304; Doyle, Anthony/0000-0001-6322-6195; spagnolo, stefania/0000-0001-7482-6348; Ferrando, James/0000-0002-1007-7816; Joergensen, Morten/0000-0002-6790-9361; Boyko, Igor/0000-0002-3355-4662; Mitsou, Vasiliki/0000-0002-1533-8886; Carquin, Edson/0000-0002-7863-1166; Mir, Lluisa-Maria/0000-0002-4276-715X; Livan, Michele/0000-0002-5877-0062; Brooks, William/0000-0001-6161-3570; Villa, Mauro/0000-0002-9181-8048; White, Ryan/0000-0003-3589-5900; Di Domenico, Antonio/0000-0001-8078-2759; Connell, Simon/0000-0001-6000-7245; Bosman, Martine/0000-0002-7290-643X; Gerbaudo, Davide/0000-0002-4463-0878; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Ventura, Andrea/0000-0002-3368-3413; Kantserov, Vadim/0000-0001-8255-416X; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Goncalo, Ricardo/0000-0002-3826-3442; Gauzzi, Paolo/0000-0003-4841-5822; Mindur, Bartosz/0000-0002-5511-2611; Fabbri, Laura/0000-0002-4002-8353; Mashinistov, Ruslan/0000-0001-7925-4676; Smirnova, Oxana/0000-0003-2517-531X; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Olshevskiy, Alexander/0000-0002-8902-1793; FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC; Belarus; CNPq; FAPESP, Brazil; NSERC; NRC; CFI, Canada FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC; Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSW', :European Union; IN2P3-CNRS, GEA-DSMARFU, France; GNSF, Georgia; BMBF, :DFG, iEIGF, MPG and Avf.1 Foundation, Germany; cs-RT and INSRF; Greece; ISF, MINERVA, GW, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and jSPS; japan; C:NRST, Morocco; FOM: and NW, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; -NIES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR; Slovakia; ARRS and MFZS, Slovenia; DST/NRF, South Africa.; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SKR, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. NR 82 TC 23 Z9 23 U1 12 U2 82 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAR 17 PY 2015 IS 3 AR 088 DI 10.1007/JHEP03(2015)088 PG 45 WC Physics, Particles & Fields SC Physics GA CD8TN UT WOS:000351369000008 ER PT J AU Chatterji, T dos Santos, AM Molaison, JJ Hansen, TC Klotz, S Tucker, M Samanta, K Saha-Dasgupta, T AF Chatterji, Tapan dos Santos, Antonio M. Molaison, Jamie J. Hansen, Thomas C. Klotz, Stefan Tucker, Mathew Samanta, Kartik Saha-Dasgupta, Tanusri TI Anomalous breakdown of Bloch's rule in the Mott-Hubbard insulator MnTe2 SO PHYSICAL REVIEW B LA English DT Article ID ANTIFERROMAGNETIC PHASE-TRANSITION; X-RAY-DIFFRACTION; HIGH-PRESSURE; MNS2; SUPEREXCHANGE; DEPENDENCE; ELECTRON; DISTANCE; PYRITE; ORDER AB We reinvestigate the pressure dependence of the crystal structure and antiferromagnetic phase transition in MnTe2 using the rigorous and reliable tool of high-pressure neutron powder diffraction. First-principles density functional theory calculations are carried out in order to gain microscopic insight. The measured Neel temperature of MnTe2 is found to show unusually large pressure dependence of 12 K GPa(-1). This gives rise to a large violation of Bloch's rule given by alpha = dlogT(N)/dlogV = -10/3 approximate to -3.3, to an alpha value of -6.0 +/- 0.1 for MnTe2. The ab initio calculation of the electronic structure and the magnetic exchange interactions in MnTe2 for the measured crystal structures at different pressures indicates the pressure dependence of the Neel temperature alpha is -5.61, in close agreement with experimental findings. The microscopic origin of this behavior turns out to be dictated by the distance dependence of the cation-anion hopping interaction strength. C1 [Chatterji, Tapan; Hansen, Thomas C.] Inst Max Von Laue Paul Langevin, F-38042 Grenoble 9, France. [dos Santos, Antonio M.; Molaison, Jamie J.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Klotz, Stefan] Univ Paris 06, CNRS, IMPMC, UMR 7590, F-75252 Paris, France. [Tucker, Mathew] Rutherford Appleton Lab, ISIS Facil, Didcot OX11 0QX, Oxon, England. [Samanta, Kartik; Saha-Dasgupta, Tanusri] SN Bose Natl Ctr Basic Sci, Dept Condensed Matter Phys & Mat Sci, Kolkata 700098, India. RP Chatterji, T (reprint author), Inst Max Von Laue Paul Langevin, Boite Postale 156, F-38042 Grenoble 9, France. RI dos Santos, Antonio/A-5602-2016; Hansen, Thomas/A-2729-2012; D20, Diffractometer/O-3123-2013; Tucker, Matt/C-9867-2016; Klotz, Stefan/D-6497-2017 OI dos Santos, Antonio/0000-0001-6900-0816; Hansen, Thomas/0000-0003-4611-2393; D20, Diffractometer/0000-0002-1572-1367; Tucker, Matt/0000-0002-2891-7086; FU Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy FX Research conducted at ORNL's Spallation Neutron Source, was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. NR 30 TC 1 Z9 1 U1 4 U2 38 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAR 17 PY 2015 VL 91 IS 10 AR 104412 DI 10.1103/PhysRevB.91.104412 PG 7 WC Physics, Condensed Matter SC Physics GA CE0QI UT WOS:000351509100001 ER PT J AU Jin, WC Yeh, PC Zaki, N Zhang, DT Liou, JT Sadowski, JT Barinov, A Yablonskikh, M Dadap, JI Sutter, P Herman, IP Osgood, RM AF Jin, Wencan Yeh, Po-Chun Zaki, Nader Zhang, Datong Liou, Jonathan T. Sadowski, Jerzy T. Barinov, Alexey Yablonskikh, Mikhail Dadap, Jerry I. Sutter, Peter Herman, Irving P. Osgood, Richard M., Jr. TI Substrate interactions with suspended and supported monolayer MoS2: Angle-resolved photoemission spectroscopy SO PHYSICAL REVIEW B LA English DT Article ID ELECTRON-MICROSCOPY; EPITAXIAL GRAPHENE; LAYER MOS2; DIFFRACTION; TRANSISTORS; BEAMLINE; SURFACE AB We report the directly measured electronic structure of exfoliated monolayer molybdenum disulfide (MoS2) using micrometer-scale angle-resolved photoemission spectroscopy. Measurements of both suspended and supported monolayer MoS2 elucidate the effects of interaction with a substrate. A suggested relaxation of the in-plane lattice constant is found for both suspended and supported monolayer MoS2 crystals. For suspended MoS2, a careful investigation of the measured uppermost valence band gives an effective mass at (Gamma) over bar and (K) over bar of 2.00m(0) and 0.43m(0), respectively. We also measure an increase in the band linewidth from the midpoint of (Gamma K) over bar to the vicinity of (K) over bar and briefly discuss its possible origin. C1 [Jin, Wencan; Yeh, Po-Chun; Zaki, Nader; Zhang, Datong; Liou, Jonathan T.; Dadap, Jerry I.; Herman, Irving P.; Osgood, Richard M., Jr.] Columbia Univ, New York, NY 10027 USA. [Sadowski, Jerzy T.; Sutter, Peter] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Barinov, Alexey; Yablonskikh, Mikhail] Elettra Sincrotrone Trieste SCpA, I-34012 Trieste, Italy. RP Osgood, RM (reprint author), Columbia Univ, New York, NY 10027 USA. EM osgood@columbia.edu OI BARINOV, Alexey/0000-0003-4125-3779; Sadowski, Jerzy/0000-0002-4365-7796 FU Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-FG 02-04-ER-46157]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886, DE-SC0012704]; 2D-materials research in the Center for Redefining Photovoltaic Efficiency through Molecular-Scale Control, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001085]; NSF MRSEC program through Columbia in the Center for Precision Assembly of Superstratic and Superatomic Solids [DMR-1420634] FX We thank Brian Souhan for making the patterned cavities on the Si substrate. We also thank Xiang Meng for useful discussions. This work was supported by the Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Award Contract No. DE-FG 02-04-ER-46157. The research is carried out in part at the Center for Functional Nanomaterials and National Synchrotron Light Source, Brookhaven National Laboratory, supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract Nos. DE-AC02-98CH10886 and DE-SC0012704. D.Z., J.T.L., and I.P.H. were supported as part of the 2D-materials research in the Center for Redefining Photovoltaic Efficiency through Molecular-Scale Control, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award No. DE-SC0001085. D.Z. and I.P.H. were also supported in part by the NSF MRSEC program through Columbia in the Center for Precision Assembly of Superstratic and Superatomic Solids (DMR-1420634). NR 36 TC 15 Z9 15 U1 4 U2 53 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAR 17 PY 2015 VL 91 IS 12 AR 121409 DI 10.1103/PhysRevB.91.121409 PG 6 WC Physics, Condensed Matter SC Physics GA CE0QS UT WOS:000351510100001 ER PT J AU Aaltonen, T Amerio, S Amidei, D Anastassov, A Annovi, A Antos, J Apollinari, G Appel, JA Arisawa, T Artikov, A Asaadi, J Ashmanskas, W Auerbach, B Aurisano, A Azfar, F Badgett, W Bae, T Barbaro-Galtieri, A Barnes, VE Barnett, BA Barria, P Bartos, P Bauce, M Bedeschi, F Behari, S Bellettini, G Bellinger, J Benjamin, D Beretvas, A Bhatti, A Bland, KR Blumenfeld, B Bocci, A Bodek, A Bortoletto, D Boudreau, J Boveia, A Brigliadori, L Bromberg, C Brucken, E Budagov, J Budd, HS Burkett, K Busetto, G Bussey, P Butti, P Buzatu, A Calamba, A Camarda, S Campanelli, M Canelli, F Carls, B Carlsmith, D Carosi, R Carrillo, S Casal, B Casarsa, M Castro, A Catastini, P Cauz, D Cavaliere, V Cerri, A Cerrito, L Chen, YC Chertok, M Chiarelli, G Chlachidze, G Cho, K Chokheli, D Clark, A Clarke, C Convery, ME Conway, J Corbo, M Cordelli, M Cox, CA Cox, DJ Cremonesi, M Cruz, D Cuevas, J Culbertson, R d'Ascenzo, N Datta, M de Barbaro, P Demortier, L Deninno, M D'Errico, M Devoto, F Di Canto, A Di Ruzza, B Dittmann, JR Donati, S D'Onofrio, M Dorigo, M Driutti, A Ebina, K Edgar, R Elagin, A Erbacher, R Errede, S Esham, B Farrington, S Ramos, JPF Field, R Flanagan, G Forrest, R Franklin, M Freeman, JC Frisch, H Funakoshi, Y Galloni, C Garfinkel, AF Garosi, P Gerberich, H Gerchtein, E Giagu, S Giakoumopoulou, V Gibson, K Ginsburg, CM Giokaris, N Giromini, P Glagolev, V Glenzinski, D Gold, M Goldin, D Golossanov, A Gomez, G Gomez-Ceballos, G Goncharov, M Lopez, OG Gorelov, I Goshaw, AT Goulianos, K Gramellini, E Grosso-Pilcher, C Group, RC da Costa, JG Hahn, SR Han, JY Happacher, F Hara, K Hare, M Harr, RF Harrington-Taber, T Hatakeyama, K Hays, C Heinrich, J Herndon, M Hocker, A Hong, Z Hopkins, W Hou, S Hughes, RE Husemann, U Hussein, M Huston, J Introzzi, G Iori, M Ivanov, A James, E Jang, D Jayatilaka, B Jeon, EJ Jindariani, S Jones, M Joo, KK Jun, SY Junk, TR Kambeitz, M Kamon, T Karchin, PE Kasmi, A Kato, Y Ketchum, W Keung, J Kilminster, B Kim, DH Kim, HS Kim, JE Kim, MJ Kim, SH Kim, SB Kim, YJ Kim, YK Kimura, N Kirby, M Knoepfel, K Kondo, K Kong, DJ Konigsberg, J Kotwal, AV Kreps, M Kroll, J Kruse, M Kuhr, T Kurata, M Laasanen, AT Lammel, S Lancaster, M Lannon, K Latino, G Lee, HS Lee, JS Leo, S Leone, S Lewis, JD Limosani, A Lipeles, E Lister, A Liu, H Liu, Q Liu, T Lockwitz, S Loginov, A Lucchesi, D Luca, A Lueck, J Lujan, P Lukens, P Lungu, G Lys, J Lysak, R Madrak, R Maestro, P Malik, S Manca, G Manousakis-Katsikakis, A Marchese, L Margaroli, F Marino, P Matera, K Mattson, ME Mazzacane, A Mazzanti, P McNulty, R Mehta, A Mehtala, P Mesropian, C Miao, T Mietlicki, D Mitra, A Miyake, H Moed, S Moggi, N Moon, CS Moore, R Morello, MJ Mukherjee, A Muller, T Murat, P Mussini, M Nachtman, J Nagai, Y Naganoma, J Nakano, I Napier, A Nett, J Neu, C Nigmanov, T Nodulman, L Noh, SY Norniella, O Oakes, L Oh, SH Oh, YD Oksuzian, I Okusawa, T Orava, R Ortolan, L Pagliarone, C Palencia, E Palni, P Papadimitriou, V Parker, W Pauletta, G Paulini, M Paus, C Phillips, TJ Piacentino, G Pianori, E Pilot, J Pitts, K Plager, C Pondrom, L Poprocki, S Potamianos, K Pranko, A Prokoshin, F Ptohos, F Punzi, G Fernandez, IR Renton, P Rescigno, M Rimondi, F Ristori, L Robson, A Rodriguez, T Rolli, S Ronzani, M Roser, R Rosner, JL Ruffini, F Ruiz, A Russ, J Rusu, V Sakumoto, WK Sakurai, Y Santi, L Sato, K Saveliev, V Savoy-Navarro, A Schlabach, P Schmidt, EE Schwarz, T Scodellaro, L Scuri, F Seidel, S Seiya, Y Semenov, A Sforza, F Shalhout, SZ Shears, T Shepard, PF Shimojima, M Shochet, M Shreyber-Tecker, I Simonenko, A Sliwa, K Smith, JR Snider, FD Song, H Sorin, V St Denis, R Stancari, M Stentz, D Strologas, J Sudo, Y Sukhanov, A Suslov, I Takemasa, K Takeuchi, Y Tang, J Tecchio, M Teng, PK Thom, J Thomson, E Thukral, V Toback, D Tokar, S Tollefson, K Tomura, T Tonelli, D Torre, S Torretta, D Totaro, P Trovato, M Ukegawa, F Uozumi, S Velev, G Vellidis, C Vernieri, C Vidal, M Vilar, R Vizan, J Vogel, M Volpi, G Vazquez, F Wagner, P Wallny, R Wang, SM Waters, D Wester, WC Whiteson, D Wicklund, AB Wilbur, S Williams, HH Wilson, JS Wilson, P Winer, BL Wittich, P Wolbers, S Wolfe, H Wright, T Wu, X Wu, Z Yamamoto, K Yamato, D Yang, T Yang, UK Yang, YC Yao, WM Yeh, GP Yi, K Yoh, J Yorita, K Yoshida, T Yu, GB Yu, I Zanetti, AM Zeng, Y Zhou, C Zucchellia, S AF Aaltonen, T. 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CA CDF Collaboration TI Search for production of an Y(1S) meson in association with a W or Z boson using the full 1.96 TeV p(p)over-bar collision data set at CDF SO PHYSICAL REVIEW D LA English DT Article ID SILICON VERTEX DETECTOR AB Production of the Y(1S) meson in association with a vector boson is a rare process in the standard model with a cross section predicted to be below the sensitivity of the Tevatron. Observation of this process could signify contributions not described by the standard model or reveal limitations with the current nonrelativistic quantum-chromodynamic models used to calculate the cross section. We perform a search for this process using the full Run II data set collected by the CDF II detector corresponding to an integrated luminosity of 9.4 fb(-1). The search considers the Y -> mu mu decay and the decay of the W and Z bosons into muons and electrons. In these purely leptonic decay channels, we observe one YW candidate with an expected background of 1.2 +/- 0.5 events, and one YZ candidate with an expected background of 0.1 +/- 0.1 events. Both observations are consistent with the predicted background contributions. The resulting upper limits on the cross section for Y + W/Z production are the most sensitive reported from a single experiment and place restrictions on potential contributions from non-standard-model physics. C1 [Chen, Y. C.; Hou, S.; Mitra, A.; Teng, P. K.; Wang, S. M.] Acad Sinica, Inst Phys, Taipei 11529, Taiwan. [Auerbach, B.; Nodulman, L.; Wicklund, A. B.] Argonne Natl Lab, Argonne, IL 60439 USA. [Giakoumopoulou, V.; Giokaris, N.; Manousakis-Katsikakis, A.] Univ Athens, GR-15771 Athens, Greece. [Camarda, S.; Ortolan, L.; Sorin, V.] Univ Autonoma Barcelona, ICREA, Inst Fis Altes Energies, E-08193 Bellaterra, Barcelona, Spain. [Bland, K. R.; Dittmann, J. 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C.; Liu, H.; Neu, C.; Oksuzian, I.] Univ Virginia, Charlottesville, VA 22906 USA. [Arisawa, T.; Ebina, K.; Funakoshi, Y.; Kimura, N.; Kondo, K.; Naganoma, J.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo 169, Japan. [Clarke, C.; Harr, R. F.; Karchin, P. E.; Mattson, M. E.] Wayne State Univ, Detroit, MI 48201 USA. [Bellinger, J.; Carlsmith, D.; Herndon, M.; Parker, W.; Pondrom, L.] Univ Wisconsin, Madison, WI 53706 USA. [Husemann, U.; Lockwitz, S.; Loginov, A.] Yale Univ, New Haven, CT 06520 USA. RP Aaltonen, T (reprint author), Univ Helsinki, Dept Phys, Div High Energy Phys, FIN-00014 Helsinki, Finland. RI vilar, rocio/P-8480-2014; Chiarelli, Giorgio/E-8953-2012; Introzzi, Gianluca/K-2497-2015; Piacentino, Giovanni/K-3269-2015; Marino, Pietro/N-7030-2015; song, hao/I-2782-2012; Gorelov, Igor/J-9010-2015; maestro, paolo/E-3280-2010; Prokoshin, Fedor/E-2795-2012; Canelli, Florencia/O-9693-2016; Ruiz, Alberto/E-4473-2011; Paulini, Manfred/N-7794-2014 OI Chiarelli, Giorgio/0000-0001-9851-4816; Introzzi, Gianluca/0000-0002-1314-2580; Piacentino, Giovanni/0000-0001-9884-2924; Marino, Pietro/0000-0003-0554-3066; song, hao/0000-0002-3134-782X; Gorelov, Igor/0000-0001-5570-0133; maestro, paolo/0000-0002-4193-1288; Prokoshin, Fedor/0000-0001-6389-5399; Canelli, Florencia/0000-0001-6361-2117; Ruiz, Alberto/0000-0002-3639-0368; Paulini, Manfred/0000-0002-6714-5787 FU U.S. Department of Energy; National Science Foundation; Italian Istituto Nazionale di Fisica Nucleare; Ministry of Education, Culture, Sports, Science and Technology of Japan; Natural Sciences and Engineering Research Council of Canada; National Science Council of the Republic of China; Swiss National Science Foundation; A. P. Sloan Foundation; Bundesministerium fur Bildung und Forschung, Germany; Korean World Class University Program, the National Research Foundation of Korea; Science and Technology Facilities Council, United Kingdom; Royal Society, United Kingdom; Russian Foundation for Basic Research; Ministerio de Ciencia e Innovacion, Spain; Programa Consolider-Ingenio, Spain; Slovak RD Agency; Academy of Finland; Australian Research Council (ARC); EU community Marie Curie Fellowship [302103] FX We would like to acknowledge K. W. Lai for suggesting the search for these processes, and thank P. Artoisenet and J.-P. Lansberg for many useful discussions and help with theoretical inputs into the MADGRAPH simulation. We thank the Fermilab staff and the technical staffs of the participating institutions for their vital contributions. This work was supported by the U.S. Department of Energy and National Science Foundation; the Italian Istituto Nazionale di Fisica Nucleare; the Ministry of Education, Culture, Sports, Science and Technology of Japan; the Natural Sciences and Engineering Research Council of Canada; the National Science Council of the Republic of China; the Swiss National Science Foundation; the A. P. Sloan Foundation; the Bundesministerium fur Bildung und Forschung, Germany; the Korean World Class University Program, the National Research Foundation of Korea; the Science and Technology Facilities Council and the Royal Society, United Kingdom; the Russian Foundation for Basic Research; the Ministerio de Ciencia e Innovacion, and Programa Consolider-Ingenio 2010, Spain; the Slovak R&D Agency; the Academy of Finland; the Australian Research Council (ARC); and the EU community Marie Curie Fellowship Contract No. 302103. NR 25 TC 2 Z9 2 U1 1 U2 19 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD MAR 17 PY 2015 VL 91 IS 5 AR 052011 DI 10.1103/PhysRevD.91.052011 PG 10 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CE0RA UT WOS:000351510900002 ER PT J AU Abazov, VM Abbott, B Acharya, BS Adams, M Adams, T Agnew, JP Alexeev, GD Alkhazov, G Alton, A Askew, A Atkins, S Augsten, K Avila, C Badaud, F Bagby, L Baldin, B Bandurin, DV Banerjee, S Barberis, E Baringer, P Bartlett, JF Bassler, U Bazterra, V Bean, A Begalli, M Bellantoni, L Beri, SB Bernardi, G Bernhard, R Bertram, I Besancon, M Beuselinck, R Bhat, PC Bhatia, S Bhatnagar, V Blazey, G Blessing, S Bloom, K Boehnlein, A Boline, D Boos, EE Borissov, G Borysova, M Brandt, A Brandt, O Brock, R Bross, A Brown, D Bu, XB Buehler, M Buescher, V Bunichev, V Burdin, S Buszello, CP Camacho-Perez, E Casey, BCK Castilla-Valdez, H Caughron, S Chakrabarti, S Chan, KM Chandra, A Chapon, E Chen, G Cho, SW Choi, S Choudhary, B Cihangir, S Claes, D Clutter, J Cooke, M Cooper, WE Corcoran, M Couderc, F Cousinou, MC Cutts, D Das, A Davies, G de Jong, SJ De la Cruz-Burelo, E Deliot, F Demina, R Denisov, D Denisov, SP Desai, S Deterre, C DeVaughan, K Diehl, HT Diesburg, M Ding, PF Dominguez, A Dubey, A Dudko, LV Duperrin, A Dutt, S Eads, M Edmunds, D Ellison, J Elvira, VD Enari, Y Evans, H Evdokimov, VN Faure, A Feng, L Ferbel, T Fiedler, F Filthaut, F Fisher, W Fisk, HE Fortner, M Fox, H Fuess, S Garbincius, PH Garcia-Bellido, A Garcia-Gonzalez, JA Gavrilov, V Geng, W Gerber, CE Gershtein, Y Ginther, G Gogota, O Golovanov, G Grannis, PD Greder, S Greenlee, H Grenier, G Gris, P Grivaz, JF Grohsjean, A Grunendahl, S Grunewald, MW Guillemin, T Gutierrez, G Gutierrez, P Haley, J Han, L Harder, K Harel, A Hauptman, JM Hays, J Head, T Hebbeker, T Hedin, D Hegab, H Heinson, AP Heintz, U Hensel, C Heredia-De La Cruz, I Herner, K Hesketh, G Hildreth, MD Hirosky, R Hoang, T Hobbs, JD Hoeneisen, B Hogan, J Hohlfeld, M Holzbauer, JL Howley, I Hubacek, Z Hynek, V Iashvili, I Ilchenko, Y Illingworth, R Ito, AS Jabeen, S Jaffre, M Jayasinghe, A Jeong, MS Jesik, R Jiang, P Johns, K Johnson, E Johnson, M Jonckheere, A Jonsson, P Joshi, J Jung, AW Juste, A Kajfasz, E Karmanov, D Katsanos, I Kaur, M Kehoe, R Kermiche, S Khalatyan, N Khanov, A Kharchilava, A Kharzheev, YN Kiselevich, I Kohli, JM Kozelov, AV Kraus, J Kumar, A Kupco, A Kurca, T Kuzmin, VA Lammers, S Lebrun, P Lee, HS Lee, SW Lee, WM Lei, X Lellouch, J Li, D Li, H Li, L Li, QZ Lim, JK Lincoln, D Linnemann, J Lipaev, VV Lipton, R Liu, H Liu, Y Lobodenko, A Lokajicek, M de Sa, RL Luna-Garcia, R Lyon, AL Maciel, AKA Madar, R Magana-Villalba, R Malik, S Malyshev, VL Mansour, J Martinez-Ortega, J McCarthy, R McGivern, CL Meijer, MM Melnitchouk, A Menezes, D Mercadante, PG Merkin, M Meyer, A Meyer, J Miconi, F Mondal, NK Mulhearn, M Nagy, E Narain, M Nayyar, R Neal, HA Negret, JP Neustroev, P Nguyen, HT Nunnemann, T Orduna, J Osman, N Osta, J Pal, A Parashar, N Parihar, V Park, SK Partridge, R Parua, N Patwa, A Penning, B Perfilov, M Peters, Y Petridis, K Petrillo, G Petroff, P Pleier, MA Podstavkov, VM Popov, AV Prewitt, M Price, D Prokopenko, N Qian, J Quadt, A Quinn, B Ratoff, PN Razumov, I Ripp-Baudot, I Rizatdinova, F Rominsky, M Ross, A Royon, C Rubinov, P Ruchti, R Sajot, G Sanchez-Hernandez, A Sanders, MP Santos, AS Savage, G Savitskyi, M Sawyer, L Scanlon, T Schamberger, RD Scheglov, Y Schellman, H Schwanenberger, C Schwienhorst, R Sekaric, J Severini, H Shabalina, E Shary, V Shaw, S Shchukin, AA Simak, V Skubic, P Slattery, P Smirnov, D Snow, GR Snow, J Snyder, S Soldner-Rembold, S Sonnenschein, L Soustruznik, K Stark, J Stoyanova, DA Strauss, M Suter, L Svoisky, P Titov, M Tokmenin, VV Tsai, YT Tsybychev, D Tuchming, B Tully, C Uvarov, L Uvarov, S Uzunyan, S Van Kooten, R van Leeuwen, WM Varelas, N Varnes, EW Vasilyev, IA Verkheev, AY Vertogradov, LS Verzocchi, M Vesterinen, M Vilanova, D Vokac, P Wahl, HD Wang, MHLS Warchol, J Watts, G Wayne, M Weichert, J Welty-Rieger, L Williams, MRJ Wilson, GW Wobisch, M Wood, DR Wyatt, TR Xie, Y Yamada, R Yang, S Yasuda, T Yatsunenko, YA Ye, W Ye, Z Yin, H Yip, K Youn, SW Yu, JM Zennamo, J Zhao, TG Zhou, B Zhu, J Zielinski, M Zieminska, D Zivkovic, L AF Abazov, V. 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Tully, C. Uvarov, L. Uvarov, S. Uzunyan, S. Van Kooten, R. van Leeuwen, W. M. Varelas, N. Varnes, E. W. Vasilyev, I. A. Verkheev, A. Y. Vertogradov, L. S. Verzocchi, M. Vesterinen, M. Vilanova, D. Vokac, P. Wahl, H. D. Wang, M. H. L. S. Warchol, J. Watts, G. Wayne, M. Weichert, J. Welty-Rieger, L. Williams, M. R. J. Wilson, G. W. Wobisch, M. Wood, D. R. Wyatt, T. R. Xie, Y. Yamada, R. Yang, S. Yasuda, T. Yatsunenko, Y. A. Ye, W. Ye, Z. Yin, H. Yip, K. Youn, S. W. Yu, J. M. Zennamo, J. Zhao, T. G. Zhou, B. Zhu, J. Zielinski, M. Zieminska, D. Zivkovic, L. CA D0 Collaboration TI Measurement of the ratio of inclusive cross sections sigma(p(p)over-bar) -> Z+2b jets/sigma(p((p)over-bar) -> Z+2 jets) in p((p)over-bar) collisions at root s=1.96 TeV SO PHYSICAL REVIEW D LA English DT Article ID D0 COLLABORATION; DETECTOR; IDENTIFICATION; P(P)OVER-BAR C1 [Hensel, C.; Maciel, A. K. A.; Santos, A. S.; Zivkovic, L.] Ctr Brasileiro Pesquisas Fis, LAFEX, Rio De Janeiro, Brazil. 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[Grivaz, J. -F.; Guillemin, T.; Jaffre, M.] Univ Paris 11, CNRS, IN2P3, LAL, F-91405 Orsay, France. [Bernardi, G.; Brown, D.; Enari, Y.; Lellouch, J.; Li, D.] Univ Paris 06, LPNHE, Paris, France. [Bernardi, G.; Brown, D.; Enari, Y.; Lellouch, J.; Li, D.] Univ Paris 07, CNRS, IN2P3, Paris, France. [Bassler, U.; Besancon, M.; Chapon, E.; Couderc, F.; Deliot, F.; Faure, A.; Grohsjean, A.; Hubacek, Z.; Royon, C.; Shary, V.; Titov, M.; Tuchming, B.; Vilanova, D.] CEA, Irfu, SPP, Saclay, France. [Greder, S.; Miconi, F.; Ripp-Baudot, I.] Univ Strasbourg, CNRS, IN2P3, IPHC, Strasbourg, France. [Grenier, G.; Kurca, T.; Lebrun, P.] Univ Lyon 1, CNRS, IN2P3, IPNL, F-69622 Villeurbanne, France. [Grenier, G.; Kurca, T.; Lebrun, P.] Univ Lyon, Lyon, France. [Hebbeker, T.; Meyer, A.; Sonnenschein, L.] Rhein Westfal TH Aachen, Phys Inst A 3, Aachen, Germany. [Bernhard, R.; Madar, R.] Univ Freiburg, Inst Phys, D-79106 Freiburg, Germany. [Brandt, A.; Mansour, J.; Meyer, J.; Quadt, A.; Shabalina, E.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Buescher, V.; Fiedler, F.; Hohlfeld, M.; Weichert, J.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Nunnemann, T.; Sanders, M. P.] Univ Munich, Munich, Germany. [Beri, S. B.; Bhatnagar, V.; Dutt, S.; Kaur, M.; Kohli, J. M.] Panjab Univ, Chandigarh 160014, India. [Choudhary, B.; Dubey, A.] Univ Delhi, Delhi 110007, India. [Acharya, B. S.; Banerjee, S.; Mondal, N. K.] Tata Inst Fundamental Res, Bombay 400005, Maharashtra, India. [Gruenewald, M. W.] Univ Coll Dublin, Dublin 2, Ireland. [Cho, S. W.; Choi, S.; Jeong, M. S.; Lee, H. S.; Lim, J. K.; Park, S. K.] Korea Univ, Korea Detector Lab, Seoul, South Korea. [Camacho-Perez, E.; Castilla-Valdez, H.; De la Cruz-Burelo, E.; Garcia-Gonzalez, J. A.; Heredia-De la Cruz, I.; Luna-Garcia, R.; Magana-Villalba, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.] CINVESTAV, Mexico City 14000, DF, Mexico. [de Jong, S. J.; Filthaut, F.; Meijer, M. M.; van Leeuwen, W. M.] Nikhef, Amsterdam, Netherlands. [de Jong, S. J.; Filthaut, F.; Meijer, M. M.] Radboud Univ Nijmegen, NL-6525 ED Nijmegen, Netherlands. [Abazov, V. M.; Alexeev, G. D.; Golovanov, G.; Kharzheev, Y. N.; Malyshev, V. L.; Tokmenin, V. V.; Verkheev, A. Y.; Vertogradov, L. S.; Yatsunenko, Y. A.] Joint Inst Nucl Res, Dubna, Russia. [Gavrilov, V.; Kiselevich, I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Boos, E. E.; Bunichev, V.; Dudko, L. V.; Karmanov, D.; Kuzmin, V. A.; Merkin, M.; Perfilov, M.] Moscow MV Lomonosov State Univ, Moscow, Russia. [Denisov, S. P.; Evdokimov, V. N.; Kozelov, A. V.; Lipaev, V. V.; Popov, A. V.; Prokopenko, N.; Razumov, I.; Shchukin, A. A.; Stoyanova, D. A.; Vasilyev, I. A.] Inst High Energy Phys, Protvino, Russia. [Alkhazov, G.; Lobodenko, A.; Neustroev, P.; Scheglov, Y.; Uvarov, L.; Uvarov, S.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Juste, A.] Inst Catalana Recerca & Estudis Avancats, Barcelona, Spain. [Buszello, C. P.] Inst Fis Altes Energies, Barcelona, Spain. [Borysova, M.; Gogota, O.; Savitskyi, M.] Uppsala Univ, Uppsala, Sweden. [Borysova, M.; Gogota, O.; Savitskyi, M.] Taras Shevchenko Natl Univ Kyiv, Kiev, Ukraine. [Bertram, I.; Borissov, G.; Burdin, S.; Fox, H.; Ratoff, P. N.; Ross, A.] Univ Lancaster, Lancaster LA1 4YB, England. [Beuselinck, R.; Davies, G.; Hays, J.; Jesik, R.; Jonsson, P.; Scanlon, T.] Univ London Imperial Coll Sci Technol & Med, London SW7 2AZ, England. [Agnew, J. P.; Deterre, C.; Ding, P. F.; Harder, K.; Head, T.; Hesketh, G.; McGivern, C. L.; Peters, Y.; Petridis, K.; Price, D.; Schwanenberger, C.; Shaw, S.; Soeldner-Rembold, S.; Suter, L.; Vesterinen, M.; Wyatt, T. R.; Zhao, T. G.] Univ Manchester, Manchester M13 9PL, Lancs, England. [Johns, K.; Lei, X.; Nayyar, R.; Varnes, E. W.] Univ Arizona, Tucson, AZ 85721 USA. [Ellison, J.; Heinson, A. P.; Joshi, J.; Li, L.] Univ Calif Riverside, Riverside, CA 92521 USA. [Adams, T.; Askew, A.; Blessing, S.; Hoang, T.; Wahl, H. D.] Florida State Univ, Tallahassee, FL 32306 USA. [Bagby, L.; Baldin, B.; Bartlett, J. F.; Bellantoni, L.; Bhat, P. C.; Boehnlein, A.; Bross, A.; Buehler, M.; Casey, B. C. K.; Cihangir, S.; Cooke, M.; Cooper, W. E.; Denisov, D.; Diesburg, M.; Elvira, V. D.; Fisk, H. E.; Fuess, S.; Garbincius, P. H.; Ginther, G.; Greenlee, H.; Gruenendahl, S.; Gutierrez, G.; Herner, K.; Illingworth, R.; Ito, A. S.; Jabeen, S.; Johnson, M.; Jonckheere, A.; Jung, A. W.; Khalatyan, N.; Li, Q. Z.; Lincoln, D.; Lipton, R.; de Sa, R. Lopes; Lyon, A. L.; Melnitchouk, A.; Penning, B.; Podstavkov, V. M.; Rominsky, M.; Rubinov, P.; Savage, G.; Verzocchi, M.; Wang, M. H. L. S.; Xie, Y.; Yamada, R.; Yasuda, T.; Ye, Z.; Yin, H.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Adams, M.; Bazterra, V.; Evdokimov, V. N.; Gerber, C. E.; Varelas, N.] Univ Illinois, Chicago, IL 60607 USA. [Blazey, G.; Eads, M.; Feng, L.; Fortner, M.; Hedin, D.; Menezes, D.; Uzunyan, S.] No Illinois Univ, De Kalb, IL 60115 USA. [Schellman, H.; Welty-Rieger, L.] Northwestern Univ, Evanston, IL 60208 USA. [Evans, H.; Lammers, S.; Parua, N.; Van Kooten, R.; Williams, M. R. J.; Zieminska, D.] Indiana Univ, Bloomington, IN 47405 USA. [Parashar, N.] Purdue Univ Calumet, Hammond, IN 46323 USA. [Chan, K. M.; Hildreth, M. D.; Osta, J.; Ruchti, R.; Smirnov, D.; Warchol, J.; Wayne, M.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Hauptman, J. M.; Lee, S. W.] Iowa State Univ, Ames, IA 50011 USA. [Baringer, P.; Bean, A.; Chen, G.; Clutter, J.; Sekaric, J.; Wilson, G. W.] Univ Kansas, Lawrence, KS 66045 USA. [Atkins, S.; Sawyer, L.; Wobisch, M.] Louisiana Tech Univ, Ruston, LA 71272 USA. [Barberis, E.; Wood, D. R.] Northeastern Univ, Boston, MA 02115 USA. [Alton, A.; Neal, H. A.; Qian, J.; Yu, J. M.; Zhou, B.; Zhu, J.] Univ Michigan, Ann Arbor, MI 48109 USA. [Brock, R.; Caughron, S.; Edmunds, D.; Fisher, W.; Geng, W.; Johnson, E.; Linnemann, J.; Schwienhorst, R.] Michigan State Univ, E Lansing, MI 48824 USA. [Bhatia, S.; Holzbauer, J. L.; Kraus, J.; Quinn, B.] Univ Mississippi, University, MS 38677 USA. [Bloom, K.; Claes, D.; DeVaughan, K.; Dominguez, A.; Katsanos, I.; Malik, S.; Snow, G. R.] Univ Nebraska, Lincoln, NE 68588 USA. [Gershtein, Y.] Rutgers State Univ, Piscataway, NJ 08855 USA. [Tully, C.] Princeton Univ, Princeton, NJ 08544 USA. [Iashvili, I.; Kharchilava, A.; Kumar, A.; Zennamo, J.] SUNY Buffalo, Buffalo, NY 14260 USA. [Demina, R.; Ferbel, T.; Garcia-Bellido, A.; Ginther, G.; Harel, A.; Petrillo, G.; Slattery, P.; Tsai, Y. -T.; Zielinski, M.] Univ Rochester, Rochester, NY 14627 USA. [Boline, D.; Chakrabarti, S.; Grannis, P. D.; Hobbs, J. D.; McCarthy, R.; Schamberger, R. D.; Tsybychev, D.; Ye, W.] SUNY Stony Brook, Stony Brook, NY 11794 USA. [Patwa, A.; Pleier, M. -A.; Snyder, S.; Yip, K.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Snow, J.] Langston Univ, Langston, OK 73050 USA. [Abbott, B.; Gutierrez, P.; Jayasinghe, A.; Severini, H.; Skubic, P.; Strauss, M.; Svoisky, P.] Univ Oklahoma, Norman, OK 73019 USA. [Haley, J.; Hegab, H.; Khanov, A.; Rizatdinova, F.] Oklahoma State Univ, Stillwater, OK 74078 USA. [Cutts, D.; Heintz, U.; Narain, M.; Parihar, V.; Partridge, R.] Brown Univ, Providence, RI 02912 USA. [Brandt, A.; Howley, I.; Pal, A.] Univ Texas Arlington, Arlington, TX 76019 USA. [Das, A.; Ilchenko, Y.; Kehoe, R.; Liu, H.] So Methodist Univ, Dallas, TX 75275 USA. [Chandra, A.; Corcoran, M.; Hogan, J.; Orduna, J.; Prewitt, M.] Rice Univ, Houston, TX 77005 USA. [Bandurin, D. V.; Hirosky, R.; Li, H.; Mulhearn, M.; Nguyen, H. T.] Univ Virginia, Charlottesville, VA 22904 USA. [Watts, G.] Univ Washington, Seattle, WA 98195 USA. RP Abazov, VM (reprint author), Joint Inst Nucl Res, Dubna, Russia. RI Sharyy, Viatcheslav/F-9057-2014; Dudko, Lev/D-7127-2012; Merkin, Mikhail/D-6809-2012; Gutierrez, Phillip/C-1161-2011; Li, Liang/O-1107-2015 OI Sharyy, Viatcheslav/0000-0002-7161-2616; Dudko, Lev/0000-0002-4462-3192; Li, Liang/0000-0001-6411-6107 FU Department of Energy (United States of America); Alternative Energies and Atomic Energy Commission (France); National Center for Scientific Research/National Institute of Nuclear and Particle Physics (France); Ministry of Education and Science of the Russian Federation (Russia); National Research Center "Kurchatov Institute" of the Russian Federation (Russia); Russian Foundation for Basic Research (Russia); National Council for the Development of Science and Technology (Brazil); Carlos Chagas Filho Foundation for the Support of Research in the State of Rio de Janeiro (Brazil); Department of Atomic Energy (India); Department of Science and Technology (India); Administrative Department of Science, Technology and Innovation (Colombia); National Council of Science and Technology (Mexico); National Research Foundation of Korea (Korea); Foundation for Fundamental Research on Matter (The Netherlands); Science and Technology Facilities Council (United Kingdom); Royal Society (United Kingdom); Ministry of Education, Youth and Sports (Czech Republic); Bundesministerium fur Bildung und Forschung (Federal Ministry of Education and Research) (Germany); Deutsche Forschungsgemeinschaft (German Research Foundation) (Germany); Science Foundation Ireland (Ireland); Swedish Research Council (Sweden); China Academy of Sciences (China); National Natural Science Foundation of China (China); Ministry of Education and Science of Ukraine (Ukraine); National Science Foundation (United States of America) FX We thank John Campbell and Doreen Wackeroth for valuable discussions, and the staffs at Fermilab and collaborating institutions, and acknowledge support from the Department of Energy and National Science Foundation (United States of America); Alternative Energies and Atomic Energy Commission and National Center for Scientific Research/National Institute of Nuclear and Particle Physics (France); Ministry of Education and Science of the Russian Federation, National Research Center "Kurchatov Institute" of the Russian Federation, and Russian Foundation for Basic Research (Russia); National Council for the Development of Science and Technology and Carlos Chagas Filho Foundation for the Support of Research in the State of Rio de Janeiro (Brazil); Department of Atomic Energy and Department of Science and Technology (India); Administrative Department of Science, Technology and Innovation (Colombia); National Council of Science and Technology (Mexico); National Research Foundation of Korea (Korea); Foundation for Fundamental Research on Matter (The Netherlands); Science and Technology Facilities Council and The Royal Society (United Kingdom); Ministry of Education, Youth and Sports (Czech Republic); Bundesministerium fur Bildung und Forschung (Federal Ministry of Education and Research) and Deutsche Forschungsgemeinschaft (German Research Foundation) (Germany); Science Foundation Ireland (Ireland); Swedish Research Council (Sweden); China Academy of Sciences and National Natural Science Foundation of China (China); and Ministry of Education and Science of Ukraine (Ukraine). NR 37 TC 0 Z9 0 U1 4 U2 18 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD MAR 17 PY 2015 VL 91 IS 5 AR 052010 DI 10.1103/PhysRevD.91.052010 PG 9 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CE0RA UT WOS:000351510900001 ER PT J AU Schaffer, R Lee, EKH Lu, YM Kim, YB AF Schaffer, Robert Lee, Eric Kin-Ho Lu, Yuan-Ming Kim, Yong Baek TI Topological Spinon Semimetals and Gapless Boundary States in Three Dimensions SO PHYSICAL REVIEW LETTERS LA English DT Article ID INSULATORS AB Recently, there has been much effort in understanding topological phases of matter with gapless bulk excitations, which are characterized by topological invariants and protected intrinsic boundary states. Here we show that topological semimetals of Majorana fermions arise in exactly solvable Kitaev spin models on a series of three-dimensional lattices. The ground states of these models are quantum spin liquids with gapless nodal spectra of bulk Majorana fermion excitations. It is shown that these phases are topologically stable as long as certain discrete symmetries are protected. The corresponding topological indices and the gapless boundary states are explicitly computed to support these results. In contrast to previous studies of noninteracting systems, the phases discussed in this work are novel examples of gapless topological phases in interacting spin systems. C1 [Schaffer, Robert; Lee, Eric Kin-Ho; Kim, Yong Baek] Univ Toronto, Dept Phys, Toronto, ON M5S 1A7, Canada. [Schaffer, Robert; Lee, Eric Kin-Ho; Kim, Yong Baek] Univ Toronto, Ctr Quantum Mat, Toronto, ON M5S 1A7, Canada. [Lu, Yuan-Ming] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Lu, Yuan-Ming] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Kim, Yong Baek] Korea Inst Adv Study, Sch Phys, Seoul 130722, South Korea. RP Schaffer, R (reprint author), Univ Toronto, Dept Phys, 100 Coll St, Toronto, ON M5S 1A7, Canada. RI Lu, Yuan-Ming/D-7554-2017 OI Lu, Yuan-Ming/0000-0001-6275-739X FU NSF [PHYS-1066293]; NSERC; CIFAR; Centre for Quantum Materials at the University of Toronto; Office of BES, Materials Sciences Division of the U.S. DOE [DE-AC02-05CH11231] FX We thank Yige Chen for discussions. Y.-M. L. and Y. B. K. acknowledge the hospitality of the Aspen Center for Physics (NSF Grant No. PHYS-1066293), where some part of this work was performed. This research was supported by the NSERC, CIFAR, and Centre for Quantum Materials at the University of Toronto (R. S., E. K.-H. L., and Y. B. K.), and by Office of BES, Materials Sciences Division of the U.S. DOE under Contract No. DE-AC02-05CH11231 (Y.-M. L.). NR 25 TC 17 Z9 17 U1 1 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 17 PY 2015 VL 114 IS 11 AR 116803 DI 10.1103/PhysRevLett.114.116803 PG 5 WC Physics, Multidisciplinary SC Physics GA CE0PU UT WOS:000351507400013 PM 25839301 ER PT J AU Eguchi, H Umemura, M Kurotani, R Fukumura, H Sato, I Kim, JH Hoshino, Y Lee, J Amemiya, N Sato, M Hirata, K Singh, DJ Masuda, T Yamamoto, M Urano, T Yoshida, K Tanigaki, K Yamamoto, M Sato, M Inoue, S Aoki, I Ishikawa, Y AF Eguchi, Haruki Umemura, Masanari Kurotani, Reiko Fukumura, Hidenobu Sato, Itaru Kim, Jeong-Hwan Hoshino, Yujiro Lee, Jin Amemiya, Naoyuki Sato, Motohiko Hirata, Kunio Singh, David J. Masuda, Takatsugu Yamamoto, Masahiro Urano, Tsutomu Yoshida, Keiichiro Tanigaki, Katsumi Yamamoto, Masaki Sato, Mamoru Inoue, Seiichi Aoki, Ichio Ishikawa, Yoshihiro TI A magnetic anti-cancer compound for magnet-guided delivery and magnetic resonance imaging SO SCIENTIFIC REPORTS LA English DT Article ID CANCER-CHEMOTHERAPY; HYDROGEN-PEROXIDE; DRUG DELIVERY; COMPLEXES; CELLS; APOPTOSIS; DNA; NANOPARTICLES; LIPOSOMES; MELANOMA AB Research on controlled drug delivery for cancer chemotherapy has focused mainly on ways to deliver existing anti-cancer drug compounds to specified targets, e.g., by conjugating them with magnetic particles or encapsulating them in micelles. Here, we show that an iron-salen, i.e., mu-oxo N, N'bis( salicylidene) ethylenediamine iron (Fe(Salen)), but not other metal salen derivatives, intrinsically exhibits both magnetic character and anti-cancer activity. X-Ray crystallographic analysis and first principles calculations based on the measured structure support this. It promoted apoptosis of various cancer cell lines, likely, via production of reactive oxygen species. In mouse leg tumor and tail melanoma models, Fe(Salen) delivery with magnet caused a robust decrease in tumor size, and the accumulation of Fe(Salen) was visualized by magnetic resonance imaging. Fe(Salen) is an anti-cancer compound with magnetic property, which is suitable for drug delivery and imaging. We believe such magnetic anti-cancer drugs have the potential to greatly advance cancer chemotherapy for new theranostics and drug-delivery strategies. C1 [Eguchi, Haruki; Umemura, Masanari; Kim, Jeong-Hwan; Ishikawa, Yoshihiro] Yokohama City Univ, Grad Sch Med, Cardiovasc Res Inst, Yokohama, Kanagawa 232, Japan. [Eguchi, Haruki] IHI Corp, Res Lab, Adv Appl Sci Dept, Yokohama, Kanagawa, Japan. [Kurotani, Reiko] Yamagata Univ, Fac Engn, Biochem Engn, Yonezawa, Yamagata 992, Japan. [Fukumura, Hidenobu] Machida Hosp, Dept Orthoped, Machida, Tokyo, Japan. [Sato, Itaru] Yokohama City Univ, Grad Sch Med, Dept Oral Surg, Yokohama, Kanagawa 232, Japan. [Kim, Jeong-Hwan] Grad Univ, Okinawa Inst Sci & Technol, Nanoparticles Design Unit, Onna Son, Japan. [Hoshino, Yujiro; Inoue, Seiichi] Yokohama Natl Univ, Grad Sch Environm & Informat Sci, Dept Environm & Nat Sci, Yokohama, Kanagawa 240, Japan. [Lee, Jin] Yokohama City Univ, Grad Sch Med, Dept Radiol, Yokohama, Kanagawa 232, Japan. [Amemiya, Naoyuki] Kyoto Univ, Grad Sch Engn, Dept Elect Engn, Kyoto, Japan. [Sato, Motohiko] Aichi Med Univ, Dept Physiol, Nagakute, Aichi 48011, Japan. [Hirata, Kunio; Yamamoto, Masaki] RIKEN, Res Infrastruct Grp, SR Life Sci Instrumentat Unit, Wako, Saitama, Japan. [Singh, David J.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN USA. [Masuda, Takatsugu] Univ Tokyo, Inst Solid State Phys, Tokyo Neutron Sci Lab, Tokai, Ibaraki, Japan. [Yamamoto, Masahiro] Konan Univ, Fac Sci & Engn, Dept Chem Funct Mol, Kobe, Hyogo, Japan. [Urano, Tsutomu] Yokohama City Univ, Grad Sch, Yokohama, Kanagawa 232, Japan. [Yoshida, Keiichiro] Yokohama City Univ, Sch Med, Dept Histol & Cell Biol, Yokohama, Kanagawa 232, Japan. [Tanigaki, Katsumi] Tohoku Univ, Grad Sch Sci, WPI AIMR, Sendai, Miyagi 980, Japan. [Tanigaki, Katsumi] Tohoku Univ, Grad Sch Sci, Dept Phys, Sendai, Miyagi 980, Japan. [Sato, Mamoru] Yokohama City Univ, Grad Sch Med Life Sci, Struct Biol Lab, Yokohama, Kanagawa 232, Japan. [Aoki, Ichio] Natl Inst Radiol Sci, Mol Imaging Ctr, Chiba 260, Japan. RP Eguchi, H (reprint author), Yokohama City Univ, Grad Sch Med, Cardiovasc Res Inst, Yokohama, Kanagawa 232, Japan. EM haruki_eguchi@ihi.co.jp; yishikaw@med.yokohama-cu.ac.jp RI Yamamoto, Masaki/B-7844-2015; Hoshino, Yujiro/N-4999-2014; Amemiya, Naoyuki/G-2549-2012; OI Yamamoto, Masaki/0000-0002-1311-1768; Hoshino, Yujiro/0000-0002-8373-8013; Amemiya, Naoyuki/0000-0002-3000-864X; Umemura, Masanari/0000-0002-1812-5720 FU Ministry of Health, Labor and Welfare; New Energy and Industrial Technology Development Organization (NEDO); Japanese Ministry of Education, Culture, Sports, Science, and Technology [22136009]; Next generation Cancer Research Promotion Project of Japan Science and Technology Center; IHI Corporation; Yokohama City University; Department of Energy, Materials Sciences and Engineering Division; Targeted Proteins Research Program of the Ministry of Education, Culture, Sports, Science and Technology; Ministry of Education, Culture FX We thank K. Otsu, S. Ono, C. Shimada, K. Kezuka, A. Makino, A. Nagasako (Yokohama City University), T. Ohata and K. Akachi (Yokohama National University), and N. Yasuda (JASRI) for their technical assistance. This work has been supported in part by grants from the Ministry of Health, Labor and Welfare (Y.I.), and the New Energy and Industrial Technology Development Organization (NEDO) (Y.I.), a Grant-in-Aid for Scientific Research on Innovative Areas (22136009) (Y.I.), a grant from the Japanese Ministry of Education, Culture, Sports, Science, and Technology (Y.I.), Next generation Cancer Research Promotion Project of Japan Science and Technology Center (P-direct) (Y.I.), IHI Corporation (H.E. and Y.I.), and a Grant for Research and Development Project from Yokohama City University (Y.I.). Work at ORNL was supported by the Department of Energy, Materials Sciences and Engineering Division (D.J.S.). Work at RIKEN was supported by the Targeted Proteins Research Program of the Ministry of Education, Culture, Sports, Science and Technology (I.H.). This work was also supported by a grant for the Platform for Drug Discovery, Informatics, and Structural Life Science from the Ministry of Education, Culture. NR 51 TC 7 Z9 7 U1 3 U2 32 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAR 17 PY 2015 VL 5 AR 9194 DI 10.1038/srep09194 PG 14 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CD6WE UT WOS:000351230000005 PM 25779357 ER PT J AU Rog, O Dernburg, AF AF Rog, Ofer Dernburg, Abby F. TI Direct Visualization Reveals Kinetics of Meiotic Chromosome Synapsis SO CELL REPORTS LA English DT Article ID CAENORHABDITIS-ELEGANS MEIOSIS; SYNAPTONEMAL COMPLEX PROTEIN; C-ELEGANS; RECOMBINATION; GENETICS AB The synaptonemal complex (SC) is a conserved protein complex that stabilizes interactions along homologous chromosomes (homologs) during meiosis. The SC regulates genetic exchanges between homologs, thereby enabling reductional division and the production of haploid gametes. Here, we directly observe SC assembly (synapsis) by optimizing methods for long-term fluorescence recording in C. elegans. We report that synapsis initiates independently on each chromosome pair at or near pairing centers-specialized regions required for homolog associations. Once initiated, the SC extends rapidly and mostly irreversibly to chromosome ends. Quantitation of SC initiation frequencies and extension rates reveals that initiation is a rate-limiting step in homolog interactions. Eliminating the dynein-driven chromosome movements that accompany synapsis severely retards SC extension, revealing a new role for these conserved motions. This work provides the first opportunity to directly observe and quantify key aspects of meiotic chromosome interactions and will enable future in vivo analysis of germline processes. C1 [Rog, Ofer; Dernburg, Abby F.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Rog, Ofer; Dernburg, Abby F.] Howard Hughes Med Inst, Chevy Chase, MD 20815 USA. [Dernburg, Abby F.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Dept Genome Dynam, Berkeley, CA 94720 USA. [Dernburg, Abby F.] Calif Inst Quantitat Biosci, Berkeley, CA 94720 USA. RP Dernburg, AF (reprint author), Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA. EM afdernburg@lbl.gov FU NIH National Center for Research Resources (NCRR); European Molecular Biology Organization Long-Term Fellowship [ALTF 564-2010]; NIH [R01 GM065591]; Howard Hughes Medical Institute FX We thank Y. Kim for purification of the SYP-2 antibody; T. Barros for help with producing Movie S10; D.J. Wynne for innovations in live-imaging technology; and S. Nakielny, Y. Mazor, J.P. Cooper, R. Heald, and members of our laboratory for discussion and critical reading of the manuscript. Some nematode strains used in this work were provided by the Caenorhabditis Genetics Center, which is funded by the NIH National Center for Research Resources (NCRR). This work was supported by a European Molecular Biology Organization Long-Term Fellowship (ALTF 564-2010) to O.R. and support to A.F.D. from the NIH (R01 GM065591) and the Howard Hughes Medical Institute. NR 27 TC 8 Z9 8 U1 0 U2 7 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 2211-1247 J9 CELL REP JI Cell Reports PD MAR 17 PY 2015 VL 10 IS 10 BP 1639 EP 1645 DI 10.1016/j.celrep.2015.02.032 PG 7 WC Cell Biology SC Cell Biology GA CD8AE UT WOS:000351316700001 ER PT J AU Sun, WH Jayaraman, S Chen, W Persson, KA Ceder, G AF Sun, Wenhao Jayaraman, Saivenkataraman Chen, Wei Persson, Kristin A. Ceder, Gerbrand TI Nucleation of metastable aragonite CaCO3 in seawater SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE nucleation; calcium carbonate; polymorphism; surface energy; solid solution-aqueous solution equilibria ID AMORPHOUS CALCIUM-CARBONATE; ELECTRON-MICROSCOPY; ENERGY CALCULATIONS; AB-INITIO; CRYSTALLIZATION; MAGNESIUM; CLUSTERS; GROWTH; THERMODYNAMICS; DISSOLUTION AB Predicting the conditions in which a compound adopts a metastable structure when it crystallizes out of solution is an unsolved and fundamental problem in materials synthesis, and one which, if understood and harnessed, could enable the rational design of synthesis pathways toward or away from metastable structures. Crystallization of metastable phases is particularly accessible via low-temperature solution-based routes, such as chimie douce and hydrothermal synthesis, but although the chemistry of the solution plays a crucial role in governing which polymorph forms, how it does so is poorly understood. Here, we demonstrate an ab initio technique to quantify thermodynamic parameters of surfaces and bulks in equilibrium with an aqueous environment, enabling the calculation of nucleation barriers of competing polymorphs as a function of solution chemistry, thereby predicting the solution conditions governing polymorph selection. We apply this approach to resolve the long-standing "calcite-aragonite problem"-the observation that calcium carbonate precipitates as the metastable aragonite polymorph in marine environments, rather than the stable phase calcite-which is of tremendous relevance to biomineralization, carbon sequestration, paleogeochemistry, and the vulnerability of marine life to ocean acidification. We identify a direct relationship between the calcite surface energy and solution Mg-Ca ion concentrations, showing that the calcite nucleation barrier surpasses that of metastable aragonite in solutions with Mg:Ca ratios consistent with modern seawater, allowing aragonite to dominate the kinetics of nucleation. Our ability to quantify how solution parameters distinguish between polymorphs marks an important step toward the ab initio prediction of materials synthesis pathways in solution. C1 [Sun, Wenhao; Jayaraman, Saivenkataraman; Ceder, Gerbrand] MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA. [Chen, Wei; Persson, Kristin A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. RP Ceder, G (reprint author), MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA. EM gceder@mit.edu RI Chen, Wei/B-3045-2012 OI Chen, Wei/0000-0002-1135-7721 FU US Department of Energy, Office of Basic Energy Sciences [DE-FG02-96ER45571, 98CH10886]; National Science Foundation Graduate Research Fellowship; Assistant Secretary for Energy Efficiency and Renewable Energy [DE-AC02-05CH11231]; US Department of Energy, Office of Basic Energy Sciences program under Grant EDCBEE FX W.S. thanks Shirley Y. Chan for helpful discussions. This work was supported by the US Department of Energy, Office of Basic Energy Sciences, under Contract DE-FG02-96ER45571, and the National Science Foundation Graduate Research Fellowship (to W.S.). Computing resources were provided by the National Energy Research Scientific Computing Center, as well as by the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the US Department of Energy, Office of Basic Energy Sciences, under Contract DE-AC02-98CH10886. Work at the Lawrence Berkeley National Laboratory was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, under Contract DE-AC02-05CH11231. The Materials Project work is supported by US Department of Energy, Office of Basic Energy Sciences program under Grant EDCBEE. NR 57 TC 19 Z9 19 U1 15 U2 96 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAR 17 PY 2015 VL 112 IS 11 BP 3199 EP 3204 DI 10.1073/pnas.1423898112 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CD4NM UT WOS:000351060000038 PM 25739963 ER PT J AU Liu, WS Kim, HS Chen, S Jie, Q Lv, B Yao, ML Ren, ZS Opeil, CP Wilson, S Chu, CW Ren, ZF AF Liu, Weishu Kim, Hee Seok Chen, Shuo Jie, Qing Lv, Bing Yao, Mengliang Ren, Zhensong Opeil, Cyril P. Wilson, Stephen Chu, Ching-Wu Ren, Zhifeng TI n-type thermoelectric material Mg2Sn0.75Ge0.25 for high power generation SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE thermoelectrics; magnesium; tin; power factor; output power ID GROUP 2-4 SEMICONDUCTORS; 5-300 DEGREES K; THERMAL-CONDUCTIVITY; SOLID-SOLUTIONS; HEAT CAPACITY; PERFORMANCE; FIGURE; MERIT; MG2SN; TELLURIDE AB Thermoelectric power generation is one of the most promising techniques to use the huge amount of waste heat and solar energy. Traditionally, high thermoelectric figure-of-merit, ZT, has been the only parameter pursued for high conversion efficiency. Here, we emphasize that a high power factor (PF) is equivalently important for high power generation, in addition to high efficiency. A new n-type Mg2Sn-based material, Mg2Sn0.75Ge0.25, is a good example to meet the dual requirements in efficiency and output power. It was found that Mg2Sn0.75Ge0.25 has an average ZT of 0.9 and PF of 52 mu W center dot cm(-1)center dot K-2 over the temperature range of 25-450 degrees C, a peak ZT of 1.4 at 450 degrees C, and peak PF of 55 mu W center dot cm(-1)center dot K-2 at 350 degrees C. By using the energy balance of one-dimensional heat flow equation, leg efficiency and output power were calculated with T-h = 400 degrees C and T-c = 50 degrees C to be of 10.5% and 6.6 W center dot cm(-2) under a temperature gradient of 150 degrees C center dot mm(-1), respectively. C1 [Liu, Weishu; Kim, Hee Seok; Chen, Shuo; Jie, Qing; Lv, Bing; Chu, Ching-Wu; Ren, Zhifeng] Univ Houston, Dept Phys, Houston, TX 77204 USA. [Liu, Weishu; Kim, Hee Seok; Chen, Shuo; Jie, Qing; Lv, Bing; Chu, Ching-Wu; Ren, Zhifeng] Univ Houston, Texas Ctr Superconduct, Houston, TX 77204 USA. [Yao, Mengliang; Ren, Zhensong; Opeil, Cyril P.; Wilson, Stephen] Boston Coll, Dept Phys, Chestnut Hill, MA 02467 USA. [Chu, Ching-Wu] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Chu, CW (reprint author), Univ Houston, Dept Phys, Houston, TX 77204 USA. EM cwchu@uh.edu; zren@uh.edu RI Chen, Shuo/H-2491-2011; Jie, Qing/N-8673-2013; Kim, Hee Seok/N-1080-2014; Liu, WeiShu/E-7098-2011 OI Chen, Shuo/0000-0002-7145-1269; Liu, WeiShu/0000-0001-8643-822X FU Solid-State Solar-Thermal Energy Conversion Center, an Energy Frontier Research Center - US Department of Energy, Office of Science, Office of Basic Energy Science [DE-SC0001299/DE-FG02-09ER46577]; Concentrated Solar Thermoelectric Power (CSP), a Department of Energy Sun Shot CSP grant [DE-EE0005806]; US Air Force Office of Scientific Research [FA9550-09-1-0656] FX This work is partially supported by Solid-State Solar-Thermal Energy Conversion Center, an Energy Frontier Research Center funded by the US Department of Energy, Office of Science, Office of Basic Energy Science under Award DE-SC0001299/DE-FG02-09ER46577 (materials synthesis and characterizations), and partially by Concentrated Solar Thermoelectric Power (CSP), a Department of Energy Sun Shot CSP grant, under Award DE-EE0005806 (leg efficiency and output power density calculation). This work is also supported in part by US Air Force Office of Scientific Research Grant FA9550-09-1-0656, the T. L. L. Temple Foundation, the John J. and Rebecca Moores Endowment, and the State of Texas through the Texas Center for Superconductivity at the University of Houston. B.L. also acknowledges the New Faculty Award by University of Houston. NR 49 TC 33 Z9 33 U1 7 U2 73 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAR 17 PY 2015 VL 112 IS 11 BP 3269 EP 3274 DI 10.1073/pnas.1424388112 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CD4NM UT WOS:000351060000050 PM 25733845 ER PT J AU Ramshaw, BJ Shekhter, A McDonald, RD Betts, JB Mitchell, JN Tobash, PH Mielke, CH Bauer, ED Migliori, A AF Ramshaw, B. J. Shekhter, Arkady McDonald, Ross D. Betts, Jon B. Mitchell, J. N. Tobash, P. H. Mielke, C. H. Bauer, E. D. Migliori, Albert TI Avoided valence transition in a plutonium superconductor SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE unconventional superconductivity; heavy fermions; quantum criticality; valence fluctuations; resonant ultrasound spectroscopy ID PHASE-TRANSITIONS; PUCOGA5; PRESSURE; CRYSTALS; HE-3 AB The d and f electrons in correlated metals are often neither fully localized around their host nuclei nor fully itinerant. This localized/itinerant duality underlies the correlated electronic states of the high-T-c cuprate superconductors and the heavy-fermion intermetallics and is nowhere more apparent than in the 5f valence electrons of plutonium. Here, we report the full set of symmetry-resolved elastic moduli of PuCoGa5-the highest T-c superconductor of the heavy fermions (T-c = 18.5 K)-and find that the bulk modulus softens anomalously over a wide range in temperature above T-c. The elastic symmetry channel in which this softening occurs is characteristic of a valence instability therefore, we identify the elastic softening with fluctuations of the plutonium 5f mixed-valence state. These valence fluctuations disappear when the superconducting gap opens at Tc, suggesting that electrons near the Fermi surface play an essential role in the mixed-valence physics of this system and that PuCoGa5 avoids a valence transition by entering the superconducting state. The lack of magnetism in PuCoGa5 has made it difficult to reconcile with most other heavy-fermion superconductors, where superconductivity is generally believed to be mediated by magnetic fluctuations. Our observations suggest that valence fluctuations play a critical role in the unusually high T-c of PuCoGa5. C1 [Ramshaw, B. J.; Shekhter, Arkady; McDonald, Ross D.; Betts, Jon B.; Mielke, C. H.; Migliori, Albert] Los Alamos Natl Lab, Natl High Magnet Field Lab, Pulsed Field Facil, Los Alamos, NM 87545 USA. [Mitchell, J. N.; Tobash, P. H.; Bauer, E. D.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Ramshaw, BJ (reprint author), Los Alamos Natl Lab, Natl High Magnet Field Lab, Pulsed Field Facil, POB 1663, Los Alamos, NM 87545 USA. EM bradramshaw@gmail.com RI Shekhter, Arkady/H-4941-2015; Mielke, Charles/S-6827-2016; OI Shekhter, Arkady/0000-0003-1550-3690; Mielke, Charles/0000-0002-2096-5411; Mitchell, Jeremy/0000-0001-7109-3505; Bauer, Eric/0000-0003-0017-1937 FU US Department of Energy, Basic Energy Sciences, Division of Materials Sciences and Engineering; Los Alamos National Laboratory (LANL) Laboratory Directed Research & Development (LDRD) Program; National Science Foundation [DMR-1157490]; State of Florida FX The authors thank A. Finkelstein, I. Fisher, Z. Fisk, L. P. Gorkov, J. Lawrence, K. A. Modic, J. Smith, and J. Thompson for helpful discussions. Work at Los Alamos National Laboratory was performed under the auspices of the US Department of Energy, Basic Energy Sciences, Division of Materials Sciences and Engineering, and the Los Alamos National Laboratory (LANL) Laboratory Directed Research & Development (LDRD) Program. This work was performed at the National High Magnetic Field Laboratory, which is supported by National Science Foundation DMR-1157490 and the State of Florida. NR 36 TC 7 Z9 7 U1 10 U2 32 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAR 17 PY 2015 VL 112 IS 11 BP 3285 EP 3289 DI 10.1073/pnas.1421174112 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CD4NM UT WOS:000351060000053 PM 25737548 ER PT J AU Dhillon, B Feau, N Aerts, AL Beauseigle, S Bernier, L Copeland, A Foster, A Gill, N Henrissat, B Herath, P LaButti, KM Levasseur, A Lindquist, EA Majoor, E Ohm, RA Pangilinan, JL Pribowo, A Saddler, JN Sakalidis, ML de Vries, RP Grigoriev, IV Goodwin, SB Tanguay, P Hamelin, RC AF Dhillon, Braham Feau, Nicolas Aerts, Andrea L. Beauseigle, Stephanie Bernier, Louis Copeland, Alex Foster, Adam Gill, Navdeep Henrissat, Bernard Herath, Padmini LaButti, Kurt M. Levasseur, Anthony Lindquist, Erika A. Majoor, Eline Ohm, Robin A. Pangilinan, Jasmyn L. Pribowo, Amadeus Saddler, John N. Sakalidis, Monique L. de Vries, Ronald P. Grigoriev, Igor V. Goodwin, Stephen B. Tanguay, Philippe Hamelin, Richard C. TI Horizontal gene transfer and gene dosage drives adaptation to wood colonization in a tree pathogen SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE poplar pathogen; tree disease; fungal genomics; Septoria canker ID SEPTORIA-MUSIVA; POPLAR CLONES; LEAF-SPOT; HYBRID POPLAR; FOREST TREES; FUNGI; CHAETOGLOBOSINS; DOMESTICATION; POPULICOLA; EXPANSION AB Some of the most damaging tree pathogens can attack woody stems, causing lesions (cankers) that may be lethal. To identify the genomic determinants of wood colonization leading to canker formation, we sequenced the genomes of the poplar canker pathogen, Mycosphaerella populorum, and the closely related poplar leaf pathogen, M. populicola. A secondary metabolite cluster unique to M. populorum is fully activated following induction by poplar wood and leaves. In addition, genes encoding hemicellulose-degrading enzymes, peptidases, and metabolite transporters were more abundant and were up-regulated in M. populorum growing on poplar wood-chip medium compared with M. populicola. The secondary gene cluster and several of the carbohydrate degradation genes have the signature of horizontal transfer from ascomycete fungi associated with wood decay and from prokaryotes. Acquisition and maintenance of the gene battery necessary for growth in woody tissues and gene dosage resulting in gene expression reconfiguration appear to be responsible for the adaptation of M. populorum to infect, colonize, and cause mortality on poplar woody stems. C1 [Dhillon, Braham; Feau, Nicolas; Beauseigle, Stephanie; Herath, Padmini; Sakalidis, Monique L.; Hamelin, Richard C.] Univ British Columbia, Dept Forest & Conservat Sci, Vancouver, BC V6T 1Z4, Canada. [Aerts, Andrea L.; Copeland, Alex; LaButti, Kurt M.; Lindquist, Erika A.; Ohm, Robin A.; Pangilinan, Jasmyn L.; Grigoriev, Igor V.] US DOE, Joint Genome Inst, Walnut Creek, CA 94598 USA. [Bernier, Louis] Univ Laval, Ctr Etud Foret, Quebec City, PQ G1V 0A6, Canada. [Foster, Adam; Tanguay, Philippe; Hamelin, Richard C.] Nat Resources Canada, Canadian Forest Serv, Laurentian Forestry Ctr, Quebec City, PQ G1V 4C7, Canada. [Gill, Navdeep] Univ British Columbia, Dept Bot, Vancouver, BC V6T 1Z4, Canada. [Henrissat, Bernard] Aix Marseille Univ, UMR Ctr Natl Rech Sci 7257, F-13288 Marseille, France. [Henrissat, Bernard] King Abdulaziz Univ, Dept Biol Sci, Jeddah 21413, Saudi Arabia. [Levasseur, Anthony] Aix Marseille Univ, IHU Mediterranee Infect, INSERM U1095, URMITE,UM63,CNRS 7278,IRD 198, F-13005 Marseille, France. [Majoor, Eline; de Vries, Ronald P.] Royal Netherlands Acad Arts & Sci, Fungal Biodivers Ctr CBS KNAW, Cent Bur Schimmelcultures, Fungal Physiol, NL-3584 CT Utrecht, Netherlands. [Majoor, Eline; de Vries, Ronald P.] Univ Utrecht, Fungal Mol Physiol, NL-3584 CT Utrecht, Netherlands. [Pribowo, Amadeus; Saddler, John N.] Univ British Columbia, Forest Prod Biotechnol & Bioenergy, Vancouver, BC V6T 1Z4, Canada. [Goodwin, Stephen B.] Purdue Univ, ARS, USDA, Crop Prod & Pest Control Res Unit, W Lafayette, IN 47907 USA. RP Feau, N (reprint author), Univ British Columbia, Dept Forest & Conservat Sci, Vancouver, BC V6T 1Z4, Canada. EM feaunico@mail.ubc.ca; Richard.Hamelin@RNCan-NRCan.gc.ca RI Sakalidis, Monique/D-5126-2011; Ohm, Robin/I-6689-2016; de Vries, Ronald/F-8125-2011; Fac Sci, KAU, Biol Sci Dept/L-4228-2013; OI Sakalidis, Monique/0000-0001-6251-7724; de Vries, Ronald/0000-0002-4363-1123; Goodwin, Stephen/0000-0001-5708-9729; Bernier, Louis/0000-0002-1789-8190 FU Genomic Research and Development Initiative of Natural Resources Canada; Genome Canada; Genome BC Project [2112]; Office of Science of the US Department of Energy [DE-AC02-05CH11231]; Netherlands Organization for Scientific Research; Netherlands Genomics Initiative [93511035] FX This work was supported by the Genomic Research and Development Initiative of Natural Resources Canada, Genome Canada, and Genome BC Project 2112. The work conducted by the US Department of Energy Joint Genome Institute was supported by the Office of Science of the US Department of Energy under Contract DE-AC02-05CH11231. E.M. was supported by a grant from The Netherlands Organization for Scientific Research and The Netherlands Genomics Initiative 93511035 (to R.P.d.V.). NR 43 TC 7 Z9 7 U1 8 U2 41 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAR 17 PY 2015 VL 112 IS 11 BP 3451 EP 3456 DI 10.1073/pnas.1424293112 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CD4NM UT WOS:000351060000081 PM 25733908 ER PT J AU Dini-Andreote, F Stegen, JC van Elsas, JD Salles, JF AF Dini-Andreote, Francisco Stegen, James C. van Elsas, Jan Dirk Salles, Joana Falcao TI Disentangling mechanisms that mediate the balance between stochastic and deterministic processes in microbial succession SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE community assembly; neutral theory; niche theory; simulation model; evolutionary niche conservatism ID SOIL BACTERIAL COMMUNITIES; PHYLOGENETIC BETA DIVERSITY; ASSEMBLY PROCESSES; RECEDING GLACIER; CENTRAL ALPS; SALT-MARSH; RHIZOSPHERE; DYNAMICS; GRADIENT; PH AB Ecological succession and the balance between stochastic and deterministic processes are two major themes within microbial ecology, but these conceptual domains have mostly developed independent of each other. Here we provide a framework that integrates shifts in community assembly processes with microbial primary succession to better understand mechanisms governing the stochastic/deterministic balance. Synthesizing previous work, we devised a conceptual model that links ecosystem development to alternative hypotheses related to shifts in ecological assembly processes. Conceptual model hypotheses were tested by coupling spatiotemporal data on soil bacterial communities with environmental conditions in a salt marsh chronosequence spanning 105 years of succession. Analyses within successional stages showed community composition to be initially governed by stochasticity, but as succession proceeded, there was a progressive increase in deterministic selection correlated with increasing sodium concentration. Analyses of community turnover among successional stages-which provide a larger spatiotemporal scale relative to within stage analyses-revealed that changes in the concentration of soil organic matter were the main predictor of the type and relative influence of determinism. Taken together, these results suggest scale-dependency in the mechanisms underlying selection. To better understand mechanisms governing these patterns, we developed an ecological simulation model that revealed how changes in selective environments cause shifts in the stochastic/deterministic balance. Finally, we propose an extended-and experimentally testable-conceptual model integrating ecological assembly processes with primary and secondary succession. This framework provides a priori hypotheses for future experiments, thereby facilitating a systematic approach to understand assembly and succession in microbial communities across ecosystems. C1 [Dini-Andreote, Francisco; van Elsas, Jan Dirk; Salles, Joana Falcao] Univ Groningen, Groningen Inst Evolutionary Life Sci, Dept Microbial Ecol, NL-9747 AG Groningen, Netherlands. [Stegen, James C.] Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99352 USA. RP Dini-Andreote, F (reprint author), Univ Groningen, Groningen Inst Evolutionary Life Sci, Dept Microbial Ecol, NL-9747 AG Groningen, Netherlands. EM f.dini.andreote@rug.nl RI Falcao Salles, Joana/A-7313-2008; Stegen, James/Q-3078-2016 OI Stegen, James/0000-0001-9135-7424 FU Netherlands Organisation for Scientific Research (NWO); Soil Biotechnology Foundation; Linus Pauling Distinguished Post-doctoral Fellowship program at PNNL FX We thank Allan Konopka, Jim Fredrickson, Steve Lindemann, and Stephanie Jurburg for critical reading of the manuscript. We also thank the Nederlandse Vereniging voor Natuurmonumenten for granting us access to the salt marsh. This research was supported by the Netherlands Organisation for Scientific Research (NWO) and the Soil Biotechnology Foundation. A portion of the research described in this paper was conducted under the Laboratory Directed Research and Development Program at Pacific Northwest National Laboratory (PNNL), a multiprogram national laboratory operated by Battelle for the US Department of Energy. J.C.S. is grateful for the support of the Linus Pauling Distinguished Post-doctoral Fellowship program at PNNL. A portion of the research was performed using Institutional Computing at PNNL. NR 56 TC 31 Z9 31 U1 42 U2 186 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAR 17 PY 2015 VL 112 IS 11 BP E1326 EP E1332 DI 10.1073/pnas.1414261112 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CD4NM UT WOS:000351060000022 PM 25733885 ER PT J AU Luo, HX Xie, WW Tao, J Inoue, H Gyenis, A Krizan, JW Yazdani, A Zhu, YM Cava, RJ AF Luo, Huixia Xie, Weiwei Tao, Jing Inoue, Hiroyuki Gyenis, Andras Krizan, Jason W. Yazdani, Ali Zhu, Yimei Cava, Robert Joseph TI Polytypism, polymorphism, and superconductivity in TaSe2-xTex SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE superconductivity; polytypism; polymorphism; dichalcogenide; charge-density wave ID CHARGE-DENSITY-WAVE; TRANSITION-METAL DICHALCOGENIDES; STRUCTURAL PROPERTIES; ELECTRICAL-PROPERTIES; NEUTRON-SCATTERING; RAMAN-SPECTROSCOPY; 2H-TASE2; 2H-NBSE2; SELENIDES; DYNAMICS AB Polymorphism in materials often leads to significantly different physical properties-the rutile and anatase polymorphs of TiO2 are a prime example. Polytypism is a special type of polymorphism, occurring in layered materials when the geometry of a repeating structural layer is maintained but the layer-stacking sequence of the overall crystal structure can be varied; SiC is an example of a material with many polytypes. Although polymorphs can have radically different physical properties, it is much rarer for polytypism to impact physical properties in a dramatic fashion. Here we study the effects of polytypism and polymorphism on the superconductivity of TaSe2, one of the archetypal members of the large family of layered dichalcogenides. We show that it is possible to access two stable polytypes and two stable polymorphs in the TaSe2-xTex solid solution and find that the 3R polytype shows a superconducting transition temperature that is between 6 and 17 times higher than that of the much more commonly found 2H polytype. The reason for this dramatic change is not apparent, but we propose that it arises either from a remarkable dependence of T-c on subtle differences in the characteristics of the single layers present or from a surprising effect of the layer-stacking sequence on electronic properties that are typically expected to be dominated by the properties of a single layer in materials of this kind. C1 [Luo, Huixia; Xie, Weiwei; Krizan, Jason W.; Cava, Robert Joseph] Princeton Univ, Dept Chem, Princeton, NJ 08544 USA. [Inoue, Hiroyuki; Gyenis, Andras; Yazdani, Ali] Princeton Univ, Joseph Henry Labs, Princeton, NJ 08544 USA. [Inoue, Hiroyuki; Gyenis, Andras; Yazdani, Ali] Princeton Univ, Dept Phys, Princeton, NJ 08544 USA. [Tao, Jing; Zhu, Yimei] Brookhaven Natl Lab, Dept Condensed Matter Phys & Mat Sci, Upton, NY 11973 USA. RP Luo, HX (reprint author), Princeton Univ, Dept Chem, Princeton, NJ 08544 USA. EM huixial@princeton.edu; rcava@princeton.edu RI Luo, huixia/A-7544-2014; Luo, Huixia/D-8467-2017; OI Luo, huixia/0000-0003-0999-6441; Luo, Huixia/0000-0003-2703-5660; Xie, Weiwei/0000-0002-5500-8195 FU Army Research Office (ARO) Multidisciplinary University Research Initiative (MURI) [FA-9550-09-1-0953]; ARO MURI [FA-9550-10-1-0553]; Department of Energy (DOE) Basic Energy Sciences (BES) [DE FG02-08ER46544]; DOE BES; Materials Sciences and Engineering Division [DE-AC02-98CH10886]; Center for Functional Nanomaterials; ARO-MURI Program [W911NF-12-1-0461]; National Science Foundation [DMR-1104612] FX This research was primarily supported by the Army Research Office (ARO) Multidisciplinary University Research Initiative (MURI) on superconductivity, Grant FA-9550-09-1-0953. ARO MURI Grant FA-9550-10-1-0553 supported the single-crystal diffraction work, and the Department of Energy (DOE) Basic Energy Sciences (BES) supported the powder diffraction refinements through Grant DE FG02-08ER46544. The electron diffraction study at Brookhaven National Laboratory was supported by the DOE BES, by the Materials Sciences and Engineering Division under Contract DE-AC02-98CH10886, and through the use of the Center for Functional Nanomaterials. The STM work was supported under the ARO-MURI Program W911NF-12-1-0461 and the National Science Foundation Grant DMR-1104612. NR 38 TC 10 Z9 10 U1 5 U2 99 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAR 17 PY 2015 VL 112 IS 11 BP E1174 EP E1180 DI 10.1073/pnas.1502460112 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CD4NM UT WOS:000351060000005 PM 25737540 ER PT J AU Lober, J Ziebert, F Aranson, IS AF Loeber, Jakob Ziebert, Falko Aranson, Igor S. TI Collisions of deformable cells lead to collective migration SO SCIENTIFIC REPORTS LA English DT Article ID SELF-POLARIZATION; SYMMETRY-BREAKING; MOTILITY; MODEL; DYNAMICS; MOTION; FORCES; PARTICLES; MECHANISM; MOVEMENT AB Collective migration of eukaryotic cells plays a fundamental role in tissue growth, wound healing and immune response. The motion, arising spontaneously or in response to chemical and mechanical stimuli, is also important for understanding life-threatening pathologies, such as cancer and metastasis formation. We present a phase-field model to describe the movement of many self-organized, interacting cells. The model takes into account the main mechanisms of cell motility - acto-myosin dynamics, as well as substrate-mediated and cell-cell adhesion. It predicts that collective cell migration emerges spontaneously as a result of inelastic collisions between neighboring cells: collisions lead to a mutual alignment of the cell velocities and to the formation of coherently-moving multi-cellular clusters. Small cell-to-cell adhesion, in turn, reduces the propensity for large-scale collective migration, while higher adhesion leads to the formation of moving bands. Our study provides valuable insight into biological processes associated with collective cell motility. C1 [Loeber, Jakob] Tech Univ Berlin, Inst Theoret Phys, D-10623 Berlin, Germany. [Ziebert, Falko] Univ Freiburg, Inst Phys, D-79104 Freiburg, Germany. [Ziebert, Falko] CNRS, Inst Charles Sadron, UPR22, F-67034 Strasbourg 2, France. [Aranson, Igor S.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Aranson, Igor S.] Northwestern Univ, Engn Sci & Appl Math, Evanston, IL 60202 USA. RP Aranson, IS (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM aronson@anl.gov FU German Science Foundation (DFG) [GRK 1558, ZI 1232/2-1]; US Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES), Materials Science and Engineering Division FX We thank Hugues Chate and Benjamin Winkler for discussions. J.L. acknowledges funding from the German Science Foundation (DFG) within the GRK 1558. F.Z. acknowledges funding from the German Science Foundation (DFG) via project ZI 1232/2-1. I.S.A. was supported by the US Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES), Materials Science and Engineering Division. The numerical work was performed on Northern Illinois University GPU cluster GAEA. NR 55 TC 22 Z9 22 U1 2 U2 31 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAR 17 PY 2015 VL 5 AR 9172 DI 10.1038/srep09172 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CD6VU UT WOS:000351229000001 PM 25779619 ER PT J AU Moissl-Eichinger, C Auerbach, AK Probst, AJ Mahnert, A Tom, L Piceno, Y Andersen, GL Venkateswaran, K Rettberg, P Barczyk, S Pukall, R Berg, G AF Moissl-Eichinger, Christine Auerbach, Anna K. Probst, Alexander J. Mahnert, Alexander Tom, Lauren Piceno, Yvette Andersen, Gary L. Venkateswaran, Kasthuri Rettberg, Petra Barczyk, Simon Pukall, Rueiger Berg, Gabriele TI Quo vadis? Microbial profiling revealed strong effects of cleanroom maintenance and routes of contamination in indoor environments SO SCIENTIFIC REPORTS LA English DT Article ID PLANETARY PROTECTION; DIVERSITY; SPACECRAFT; BACTERIA; COMMUNITIES; ROOMS; SEQUENCES; ARCHAEA; RESISTANCE; TAXONOMY AB Space agencies maintain highly controlled cleanrooms to ensure the demands of planetary protection. To study potential effects of microbiome control, we analyzed microbial communities in two particulate-controlled cleanrooms (ISO 5 and ISO 8) and two vicinal uncontrolled areas (office, changing room) by cultivation and 16S rRNA gene amplicon analysis (cloning, pyrotagsequencing, and PhyloChip G3 analysis). Maintenance procedures affected the microbiome on total abundance and microbial community structure concerning richness, diversity and relative abundance of certain taxa. Cleanroom areas were found to be mainly predominated by potentially human-associated bacteria; archaeal signatures were detected in every area. Results indicate that microorganisms were mainly spread from the changing room (68%) into the cleanrooms, potentially carried along with human activity. The numbers of colony forming units were reduced by up to similar to 400 fold from the uncontrolled areas towards the ISO 5 cleanroom, accompanied with a reduction of the living portion of microorganisms from 45% (changing area) to 1% of total 16S rRNA gene signatures as revealed via propidium monoazide treatment of the samples. Our results demonstrate the strong effects of cleanroom maintenance on microbial communities in indoor environments and can be used to improve the design and operation of biologically controlled cleanrooms. C1 [Moissl-Eichinger, Christine; Auerbach, Anna K.; Probst, Alexander J.] Univ Regensburg, Inst Microbiol, D-93053 Regensburg, Germany. [Moissl-Eichinger, Christine; Auerbach, Anna K.; Probst, Alexander J.] Univ Regensburg, Archaea Ctr, D-93053 Regensburg, Germany. [Moissl-Eichinger, Christine] Med Univ Graz, Dept Internal Med, A-8036 Graz, Austria. [Moissl-Eichinger, Christine] BioTechMed Graz, A-8010 Graz, Austria. [Mahnert, Alexander; Berg, Gabriele] Graz Univ Technol, Inst Environm Biotechnol, A-8010 Graz, Austria. [Tom, Lauren; Piceno, Yvette; Andersen, Gary L.] Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA USA. [Venkateswaran, Kasthuri] Jet Prop Lab, Pasadena, CA 91109 USA. [Rettberg, Petra; Barczyk, Simon] German Aerosp Ctr, Inst Aerosp Med & Radiat Biol, D-51147 Cologne, Germany. [Pukall, Rueiger] DSMZ Deutsch Sammlung Mikroorganismen & Zellkult, Leibniz Inst, D-38124 Braunschweig, Germany. RP Moissl-Eichinger, C (reprint author), Univ Regensburg, Inst Microbiol, Univ Str 31, D-93053 Regensburg, Germany. EM christine.moissl-eichinger@medunigraz.at RI Tom, Lauren/E-9739-2015; Moissl-Eichinger, Christine/A-6682-2015; Piceno, Yvette/I-6738-2016; Andersen, Gary/G-2792-2015; Rettberg, Petra/K-2378-2015; Probst, Alexander/K-2813-2016 OI Moissl-Eichinger, Christine/0000-0001-6755-6263; Piceno, Yvette/0000-0002-7915-4699; Andersen, Gary/0000-0002-1618-9827; Rettberg, Petra/0000-0003-4439-2395; FU German National Academic Foundation (Studienstiftung des deutschen Volkes); ESTEC [20234/06/NL/EK, 20508/07/NL/EK, 4000103794/11/NL/EK] FX The work described in this paper was carried out by DLR and University of Regensburg under contract with ESA, ESTEC contract no. 20234/06/NL/EK, 20508/07/NL/EK and mainly 4000103794/11/NL/EK. We thank G. Bose and B. Vogt for sampling support at the Airbus/EADS facilities and T. Dohr for rendering the 3D-model of the cleanroom facility. We also would like to thank H. Muller (Graz) for bioinformatic support. AJP was supported by the German National Academic Foundation (Studienstiftung des deutschen Volkes). We thank G. Kminek for valuable discussion and support. NR 54 TC 6 Z9 6 U1 3 U2 12 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAR 17 PY 2015 VL 5 AR 9156 DI 10.1038/srep09156 PG 13 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CD6VP UT WOS:000351228500004 PM 25778463 ER PT J AU de Jong, M Chen, W Angsten, T Jain, A Notestine, R Gamst, A Sluiter, M Ande, CK van der Zwaag, S Plata, JJ Toher, C Curtarolo, S Ceder, G Persson, KA Asta, M AF de Jong, Maarten Chen, Wei Angsten, Thomas Jain, Anubhav Notestine, Randy Gamst, Anthony Sluiter, Marcel Ande, Chaitanya Krishna van der Zwaag, Sybrand Plata, Jose J. Toher, Cormac Curtarolo, Stefano Ceder, Gerbrand Persson, Kristin A. Asta, Mark TI Charting the complete elastic properties of inorganic crystalline compounds SO SCIENTIFIC DATA LA English DT Article ID INTERMETALLIC COMPOUNDS; THERMAL-CONDUCTIVITY; SINGLE-CRYSTALS; HIGH-THROUGHPUT; CONSTANTS; TRANSITION; OXIDE; 1ST-PRINCIPLES; STABILITY; SOLIDS AB The elastic constant tensor of an inorganic compound provides a complete description of the response of the material to external stresses in the elastic limit. It thus provides fundamental insight into the nature of the bonding in the material, and it is known to correlate with many mechanical properties. Despite the importance of the elastic constant tensor, it has been measured for a very small fraction of all known inorganic compounds, a situation that limits the ability of materials scientists to develop new materials with targeted mechanical responses. To address this deficiency, we present here the largest database of calculated elastic properties for inorganic compounds to date. The database currently contains full elastic information for 1,181 inorganic compounds, and this number is growing steadily. The methods used to develop the database are described, as are results of tests that establish the accuracy of the data. In addition, we document the database format and describe the different ways it can be accessed and analyzed in efforts related to materials discovery and design. C1 [de Jong, Maarten; Angsten, Thomas; Asta, Mark] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Chen, Wei; Jain, Anubhav; Persson, Kristin A.] Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Notestine, Randy; Gamst, Anthony] Univ Calif San Diego, San Diego Supercomp Ctr, Computat & Appl Stat Lab, San Diego, CA 92093 USA. [Sluiter, Marcel] Delft Univ Technol, Dept Mat Sci 3ME, NL-2628 CD Delft, Netherlands. [Ande, Chaitanya Krishna] Eindhoven Univ Technol, Dept Appl Phys, NL-5600 MB Eindhoven, Netherlands. [van der Zwaag, Sybrand] Delft Univ Technol, Dept Aerosp Engn, NL-2629 HS Delft, Netherlands. [Plata, Jose J.; Toher, Cormac] Duke Univ, Dept Mech Engn & Mat Sci, Ctr Mat Genom, Durham, NC 27708 USA. [Curtarolo, Stefano] Duke Univ, Ctr Mat Genom Mat Sci Elect Engn Phys & Chem, Durham, NC 27708 USA. [Ceder, Gerbrand] MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA. RP de Jong, M (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. EM maartendft@gmail.com RI Sluiter, Marcel/E-6086-2010; Chen, Wei/B-3045-2012 OI Sluiter, Marcel/0000-0002-6514-4318; Chen, Wei/0000-0002-1135-7721 FU BES DOE Grant [EDCBEE]; Assistant Secretary for Energy Efficiency and Renewable Energy [DE-AC02-05CH11231]; Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was intellectually led by the Materials Project Center, supported by the BES DOE Grant No. EDCBEE. Work at the Lawrence Berkeley National Laboratory was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, under Contract No. DE-AC02-05CH11231. This work made use of resources of the National Energy Research Scientific Computing Center (NERSC), supported by the Office of Basic Energy Sciences of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 79 TC 12 Z9 12 U1 2 U2 20 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2052-4463 J9 SCI DATA JI Sci. Data PD MAR 17 PY 2015 VL 2 AR UNSP 150009 DI 10.1038/sdata.2015.9 PG 13 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA EF4VA UT WOS:000390328900001 PM 25984348 ER PT J AU Fennell, JF Claudepierre, SG Blake, JB O'Brien, TP Clemmons, JH Baker, DN Spence, HE Reeves, GD AF Fennell, J. F. Claudepierre, S. G. Blake, J. B. O'Brien, T. P. Clemmons, J. H. Baker, D. N. Spence, H. E. Reeves, G. D. TI Van Allen Probes show that the inner radiation zone contains no MeV electrons: ECT/MagEIS data SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE inner radiation belt; inner zone; trapped electrons; inner magnetosphere; Van Allen Probes ID BELT; DIFFUSION AB We present Van Allen Probe observations of electrons in the inner radiation zone. The measurements were made by the Energetic Particle, Composition, and Thermal Plasma/Magnetic Electron Ion Spectrometer (MagEIS) sensors that were designed to measure electrons with the ability to remove unwanted signals from penetrating protons, providing clean measurements. No electrons >900keV were observed with equatorial fluxes above background (i.e., >0.1el/(cm(2)ssrkeV)) in the inner zone. The observed fluxes are compared to the AE9 model and CRRES observations. Electron fluxes <200keV exceeded the AE9 model 50% fluxes and were lower than the higher-energy model fluxes. Phase space density radial profiles for 1.3L*<2.5 had mostly positive gradients except near L*similar to 2.1, where the profiles for =20-30MeV/G were flat or slightly peaked. The major result is that MagEIS data do not show the presence of significant fluxes of MeV electrons in the inner zone while current radiation belt models and previous publications do. C1 [Fennell, J. F.; Claudepierre, S. G.; Blake, J. B.; O'Brien, T. P.; Clemmons, J. H.] Aerosp Corp, Space Sci Applicat Lab, El Segundo, CA 90245 USA. [Baker, D. N.] Univ Colorado, Lab Atmospher & Space Phys, Boulder, CO 80309 USA. [Spence, H. E.] Univ New Hampshire, Inst Study Earth Oceans & Space, Durham, NH 03824 USA. [Reeves, G. D.] Los Alamos Natl Lab, Los Alamos, NM USA. RP Fennell, JF (reprint author), Aerosp Corp, Space Sci Applicat Lab, El Segundo, CA 90245 USA. EM joseph.fennell@aero.org RI Reeves, Geoffrey/E-8101-2011; OI Reeves, Geoffrey/0000-0002-7985-8098; Clemmons, James/0000-0002-5298-5222 FU Van Allen Probes ECT by JHU/APL under NASA [967399, NAS5-01072]; United States Department of Energy [NNG07EK09I] FX This work was supported by Van Allen Probes ECT funding provided by JHU/APL contract 967399 under NASA's Prime contract NAS5-01072. Work at Los Alamos National Laboratory was performed under the auspices of the United States Department of Energy under Interagency Purchase Request NNG07EK09I. NR 34 TC 30 Z9 30 U1 3 U2 14 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD MAR 16 PY 2015 VL 42 IS 5 BP 1283 EP 1289 DI 10.1002/2014GL062874 PG 7 WC Geosciences, Multidisciplinary SC Geology GA CE5CL UT WOS:000351847600001 ER PT J AU Cavanaugh, NR Gershunov, A Panorska, AK Kozubowski, TJ AF Cavanaugh, Nicholas R. Gershunov, Alexander Panorska, Anna K. Kozubowski, Tomasz J. TI The probability distribution of intense daily precipitation SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE extreme; Pareto; probability; precipitation; weather station ID EXTREME ORDER-STATISTICS; DAILY RAINFALL; CLIMATE-CHANGE; UNITED-STATES; MODELS; TRENDS; TAILS; TEMPERATURE; VARIABILITY; RECORD AB The probability tail structure of over 22,000 weather stations globally is examined in order to identify the physically and mathematically consistent distribution type for modeling the probability of intense daily precipitation and extremes. Results indicate that when aggregating data annually, most locations are to be considered heavy tailed with statistical significance. When aggregating data by season, it becomes evident that the thickness of the probability tail is related to the variability in precipitation causing events and thus that the fundamental cause of precipitation volatility is weather diversity. These results have both theoretical and practical implications for the modeling of high-frequency climate variability worldwide. C1 [Cavanaugh, Nicholas R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Cavanaugh, Nicholas R.; Gershunov, Alexander] Univ Calif San Diego, Scripps Inst Oceanog, Climate Atmospher Sci & Phys Oceanog Div, La Jolla, CA 92093 USA. [Panorska, Anna K.; Kozubowski, Tomasz J.] Univ Nevada, Dept Math & Stat, Reno, NV 89557 USA. RP Cavanaugh, NR (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. EM nrcavanaugh@lbl.gov FU NSF [ATM-0236898, OCE0960770, OCE1419306]; California Climate Change Center - California Energy Commission's Public Interest Energy Research Program; NOAA Office of Global Programs under the California and Nevada Applications Program; Department of the Interior via the Southwest Climate Science Center FX This work was initially supported through NSF grant ATM-0236898 "Modeling, variability and predictability of North American hydrologic extremes." Cavanaugh was supported in part by NSF grants OCE0960770 and OCE1419306. We would like to thank J. Fein for his personal encouragement of this work. Funding was also provided by the California Climate Change Center, sponsored by the California Energy Commission's Public Interest Energy Research Program, by the NOAA Office of Global Programs, under the California and Nevada Applications Program, and by the Department of the Interior via the Southwest Climate Science Center. GHCN-D data are freely available from NOAA NCDC. The authors thank Jonathan Woody and two anonymous reviewers for their helpful comments. NR 47 TC 6 Z9 6 U1 4 U2 26 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD MAR 16 PY 2015 VL 42 IS 5 BP 1560 EP 1567 DI 10.1002/2015GL063238 PG 8 WC Geosciences, Multidisciplinary SC Geology GA CE5CL UT WOS:000351847600038 ER PT J AU Jardine, AB Jardine, KJ Fuentes, JD Martin, ST Martins, G Durgante, F Carneiro, V Higuchi, N Manzi, AO Chambers, JQ AF Jardine, A. B. Jardine, K. J. Fuentes, J. D. Martin, S. T. Martins, G. Durgante, F. Carneiro, V. Higuchi, N. Manzi, A. O. Chambers, J. Q. TI Highly reactive light-dependent monoterpenes in the Amazon SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE secondary organic aerosols; vertical forest structure; ozonolysis; atmospheric oxidation; light-dependent monoterpenes; tropical VOC emissions ID ORGANIC-COMPOUND EMISSIONS; RAIN-FOREST; OXIDATION-PRODUCTS; PHASE CHEMISTRY; GLOBAL CLIMATE; ABIOTIC STRESS; BOUNDARY-LAYER; COMPOUNDS VOC; ISOPRENE; AEROSOLS AB Despite orders of magnitude difference in atmospheric reactivity and great diversity in biological functioning, little is known about monoterpene speciation in tropical forests. Here we report vertically resolved ambient air mixing ratios for 12 monoterpenes in a central Amazon rainforest including observations of the highly reactive cis--ocimene (160ppt), trans--ocimene (79ppt), and terpinolene (32ppt) which accounted for an estimated 21% of total monoterpene composition yet 55% of the upper canopy monoterpene ozonolysis rate. All 12 monoterpenes showed a mixing ratio peak in the upper canopy, with three demonstrating subcanopy peaks in 7 of 11 profiles. Leaf level emissions of highly reactive monoterpenes accounted for up to 1.9% of photosynthesis confirming light-dependent emissions across several Amazon tree genera. These results suggest that highly reactive monoterpenes play important antioxidant roles during photosynthesis in plants and serve as near-canopy sources of secondary organic aerosol precursors through atmospheric photooxidation via ozonolysis. C1 [Jardine, A. B.; Martins, G.; Durgante, F.; Carneiro, V.; Higuchi, N.; Manzi, A. O.] Inst Nacl de Pesquisas da Amazonia, Climate & Environm Dept, Manaus, Amazonas, Brazil. [Jardine, K. J.; Chambers, J. Q.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Climate Sci Dept, Berkeley, CA 94720 USA. [Fuentes, J. D.] Penn State Univ, Dept Meteorol, Coll Earth & Mineral Sci, University Pk, PA 16802 USA. [Martin, S. T.] Harvard Univ, Sch Engn & Appl Sci, Cambridge, MA 02138 USA. [Martin, S. T.] Harvard Univ, Dept Earth & Planetary Sci, Cambridge, MA 02138 USA. [Chambers, J. Q.] Univ Calif Berkeley, Dept Geog, Berkeley, CA 94720 USA. RP Jardine, AB (reprint author), Inst Nacl de Pesquisas da Amazonia, Climate & Environm Dept, Manaus, Amazonas, Brazil. EM angela.jardine@inpa.gov.br RI Chambers, Jeffrey/J-9021-2014; Martin, Scot/G-1094-2015; Jardine, Kolby/N-2802-2013 OI Chambers, Jeffrey/0000-0003-3983-7847; Martin, Scot/0000-0002-8996-7554; Jardine, Kolby/0000-0001-8491-9310 FU Office of Science, Office of Biological and Environmental Research of the U.S. Department of Energy [DE-AC02-05CH11231]; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq) FX This research was supported by the Director, Office of Science, Office of Biological and Environmental Research of the U.S. Department of Energy under contract DE-AC02-05CH11231 as part of their Terrestrial Ecosystem Science Program. Additional funding for this research was provided in Brazil by the Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq). We would also like to thank Ana Paula Florentino for her consultation and assistance in collecting leaf level data. All data necessary to understand, evaluate, replicate, and build upon the research reported here will be curated for 5 years and will be available upon request of the corresponding author. NR 60 TC 9 Z9 10 U1 3 U2 28 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD MAR 16 PY 2015 VL 42 IS 5 BP 1576 EP 1583 DI 10.1002/2014GL062573 PG 8 WC Geosciences, Multidisciplinary SC Geology GA CE5CL UT WOS:000351847600040 ER PT J AU Mechem, DB Giangrande, SE Wittman, CS Borque, P Toto, T Kollias, P AF Mechem, David B. Giangrande, Scott E. Wittman, Carly S. Borque, Paloma Toto, Tami Kollias, Pavlos TI Insights from modeling and observational evaluation of a precipitating continental cumulus event observed during the MC3E field campaign SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article DE MC3E; cumulus; congestus; LES; cloud radar; variational analysis ID RADIATION MEASUREMENT PROGRAM; HIGH-RESOLUTION SIMULATION; CLIMATE RESEARCH FACILITY; LARGE-EDDY SIMULATIONS; MARINE BOUNDARY-LAYER; ATMOSPHERIC RADIATION; SHALLOW CUMULUS; DEEP CONVECTION; TROPICAL CONVECTION; CLOUD FRACTION AB A case of shallow cumulus and precipitating cumulus congestus sampled at the Atmospheric Radiation Measurement Program Southern Great Plains supersite during the Midlatitude Continental Convective Clouds Experiment is analyzed using a multisensor observational approach and numerical simulation. Observations from a new radar suite surrounding the facility are used to characterize the evolving statistical behavior of the precipitating cloud system. This is accomplished using distributions of different measures of cloud geometry and precipitation properties. Large-eddy simulation (LES) with size-resolved (bin) microphysics is employed to determine the forcings most important in producing the salient aspects of the cloud system captured in the radar observations. Our emphasis is on assessing the importance of time-varying versus steady state large-scale forcing on the model's ability to reproduce the evolutionary behavior of the cloud system. Additional consideration is given to how the characteristic spatial scale and homogeneity of the forcing imposed on the simulation influences the evolution of cloud system properties. Results indicate that several new scanning radar estimates such as distributions of cloud top are useful to differentiate the value of time-varying (or at least temporally well-matched) forcing on LES solution fidelity. C1 [Mechem, David B.; Wittman, Carly S.] Univ Kansas, Dept Geog, Atmospher Sci Program, Lawrence, KS 66045 USA. [Giangrande, Scott E.; Toto, Tami] Brookhaven Natl Lab, Upton, NY 11973 USA. [Borque, Paloma; Kollias, Pavlos] McGill Univ, Dept Atmospher & Ocean Sci, Montreal, PQ, Canada. RP Mechem, DB (reprint author), Univ Kansas, Dept Geog, Atmospher Sci Program, Lawrence, KS 66045 USA. EM dmechem@ku.edu RI Measurement, Global/C-4698-2015; Giangrande, Scott/I-4089-2016 OI Giangrande, Scott/0000-0002-8119-8199 FU Department of Energy Office of Science [DE-SC0006736]; U.S. National Oceanic and Atmospheric Administration (NOAA) Climate Program Office (CPO) Climate Prediction Program for the Americas/Earth System Science Program (CPPA/ESS) [NA10OAR4310160]; Office of Naval Research [N00014-11-1-0518]; U.S. Department of Energy [DE-AC02-98CH10886] FX The authors wish to thank the ARM Climate Research Facility for the extended data set collection and maintenance during the MC3E campaign period. We would like to thank Michael Jensen (BNL) for comments on a draft of the manuscript and three anonymous reviewers for constructive comments. We are grateful to Marat Khairoutdinov formaking SAM available to the scientific community and to Yefim Kogan for ongoing collaborations with the bin microphysics component of the model. Some of the computing for this project was performed at the OU Supercomputing Center for Education and Research. Beth Tully refined Figure 2. Observational data are available from the U.S. Department of Energy SGP ARM Climate Research Facility (http://www.archive.arm.gov) and the corresponding website for the Midlatitude Continental Convective Clouds Experiment (MC3E, http://campaign.arm.gov/mc3e/). Numerical simulation data are available on request of the corresponding author (dmechem@ku.edu), in accordance with AGU guidelines. This research was supported by the Department of Energy Office of Science grant DE-SC0006736, the U.S. National Oceanic and Atmospheric Administration (NOAA) Climate Program Office (CPO) Climate Prediction Program for the Americas/Earth System Science Program (CPPA/ESS) grant NA10OAR4310160, and the Office of Naval Research award N00014-11-1-0518. This manuscript has been authored by employees of Brookhaven Science Associates, LLC under contract DE-AC02-98CH10886 with the U.S. Department of Energy. The publisher by accepting the manuscript for publication acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. NR 76 TC 1 Z9 1 U1 1 U2 5 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD MAR 16 PY 2015 VL 120 IS 5 BP 1980 EP 1995 DI 10.1002/2014JD022255 PG 16 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA CE2VL UT WOS:000351678100022 ER PT J AU White, MA Cerqueira, AB Whitman, CA Johnson, MB Ogitsu, T AF White, Mary Anne Cerqueira, Anthony B. Whitman, Catherine A. Johnson, Michel B. Ogitsu, Tadashi TI Determination of Phase Stability of Elemental Boron SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE boron; phase diagrams; phase stability; structure; thermodynamics ID BETA-RHOMBOHEDRAL BORON; CRYSTAL-STRUCTURE; HIGH-PRESSURE; FORM AB Boron is an important element, used in applications from superhard materials to superconductors. Boron exists in several forms (allotropes) and, surprisingly, it was not known which form (alpha or beta) is stable at ambient conditions. Through experiment, we quantify the relative stability of alpha-boron and beta-boron as a function of temperature. The ground-state energies of alpha-boron and beta-boron are nearly identical. For all temperatures up to 2000 K, the complicated beta-boron structure is more stable than the simpler alpha-boron structure at ambient pressure. Below 1000 K, beta-boron is entropically stabilized with respect to alpha-boron owing to its partially occupied sites, whereas at higher temperatures beta-boron is enthalpically stabilized with respect to alpha-boron. We show that alpha-boron only becomes stable on application of pressure. C1 [White, Mary Anne; Cerqueira, Anthony B.; Whitman, Catherine A.; Johnson, Michel B.] Dalhousie Univ, Dept Chem, Halifax, NS B3H 4R2, Canada. [White, Mary Anne; Cerqueira, Anthony B.; Whitman, Catherine A.; Johnson, Michel B.] Dalhousie Univ, Inst Mat Res, Halifax, NS B3H 4R2, Canada. [Ogitsu, Tadashi] Lawrence Livermore Natl Lab, Condensed Matter & Mat Div, Livermore, CA 94550 USA. RP White, MA (reprint author), Dalhousie Univ, Dept Chem, Halifax, NS B3H 4R2, Canada. EM mary.anne.white@dal.ca RI White, Mary Anne/B-6479-2009 FU NSERC; Dalhousie University's Institute for Research in Materials and its Facilities for Materials Characterization; U.S. Department of Energy by the Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX We acknowledge the support of NSERC, and Dalhousie University's Institute for Research in Materials and its Facilities for Materials Characterization. We thank A. George, A. Bent, A. Becke, C. Romao, J. Niven, J. Noel, J. Pohls, P. Scallion, and T. Letcher for assistance and input. The work of T.O. was performed under the auspices of the U.S. Department of Energy by the Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 27 TC 7 Z9 7 U1 4 U2 36 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD MAR 16 PY 2015 VL 54 IS 12 BP 3626 EP 3629 DI 10.1002/anie.201409169 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA CD6DA UT WOS:000351178300012 PM 25619645 ER PT J AU Ashraf, A Dissanayake, DMNM Eisaman, MD AF Ashraf, A. Dissanayake, D. M. N. M. Eisaman, M. D. TI Measuring charge carrier mobility in photovoltaic devices with micron-scale resolution SO APPLIED PHYSICS LETTERS LA English DT Article ID HETEROJUNCTION SOLAR-CELLS; CONJUGATED POLYMER-FILMS; C-SI-H; MICROCRYSTALLINE SILICON; TRANSPORT; POLY(3-HEXYLTHIOPHENE); RECOMBINATION; EXTRACTION; AMBIPOLAR; BLENDS AB We present a charge-extraction technique, micron-scale charge extraction by linearly increasing voltage, which enables simultaneous spatially resolved measurements of charge carrier mobility and photocurrent in thin-film photovoltaic devices with micron-scale resolution. An intensity-modulated laser with beam diameter near the optical diffraction limit is scanned over the device, while a linear voltage ramp in reverse bias is applied at each position of illumination. We calculate the majority carrier mobility, photocurrent, and number of photogenerated charge carriers from the resulting current transient. We demonstrate this technique on an organic photovoltaic device, but it is applicable to a wide range of photovoltaic materials. (C) 2015 AIP Publishing LLC. C1 [Ashraf, A.; Dissanayake, D. M. N. M.; Eisaman, M. D.] Brookhaven Natl Lab, Sustainable Energy Technol Dept, Upton, NY 11973 USA. [Ashraf, A.; Eisaman, M. D.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Eisaman, M. D.] SUNY Stony Brook, Dept Elect & Comp Engn, Stony Brook, NY 11794 USA. RP Eisaman, MD (reprint author), Brookhaven Natl Lab, Sustainable Energy Technol Dept, Upton, NY 11973 USA. EM meisaman@bnl.gov FU U.S. Department of Energy, Sustainable Energy Technologies Department [DE-AC02-98CH10886]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX This work was partially supported by the U.S. Department of Energy, Sustainable Energy Technologies Department under Contract No. DE-AC02-98CH10886. Research was carried out in part at the Center for Functional Nanomaterials, Brookhaven National Laboratory, which was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. NR 27 TC 0 Z9 0 U1 1 U2 22 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAR 16 PY 2015 VL 106 IS 11 AR 113504 DI 10.1063/1.4915614 PG 5 WC Physics, Applied SC Physics GA CE1TS UT WOS:000351595500054 ER PT J AU Chen, AP Poudyal, N Xiong, J Liu, JP Jia, QX AF Chen, Aiping Poudyal, Narayan Xiong, Jie Liu, J. Ping Jia, Quanxi TI Modification of structure and magnetic anisotropy of epitaxial CoFe2O4 films by hydrogen reduction SO APPLIED PHYSICS LETTERS LA English DT Article ID PULSED-LASER DEPOSITION; THIN-FILMS AB Heteroepitaxial CoFe2O4 (CFO) thin films with different thicknesses were deposited on MgO (001) substrates. The as-deposited CFO films show a clear switching of magnetic anisotropy with increasing film thickness. The thinner films (< 100 nm) show a perpendicular magnetic anisotropy due to the out-of-plane compressive strain. The thicker films exhibit an in-plane easy axis owing to the dominating shape anisotropy effect. The magnetostriction coefficient of CFO films is estimated to be lambda([001]) = -188 x 10(-6). Metallic CoFe2 films were obtained by annealing the as-deposited CFO films in forming gas (Ar 93% + H-2 7%) at 450 degrees C. XRD shows that CoFe2 films are textured out-of-plane and aligned in-plane, owing to lattice matching between CoFe2 and MgO substrate. TEM results indicate that as-deposited films are continuous while the annealed films exhibit a nanopore mushroom structure. The magnetic anisotropy of CoFe2 films is dominated by the shape effect. The results demonstrate that hydrogen reduction can be effectively used to modify microstructures and physical properties of complex metal oxide materials. (C) 2015 AIP Publishing LLC. C1 [Chen, Aiping; Xiong, Jie; Jia, Quanxi] Los Alamos Natl Lab, Ctr Integrated Nanotechnol CINT, Los Alamos, NM 87545 USA. [Poudyal, Narayan; Liu, J. Ping] Univ Texas Arlington, Dept Phys, Arlington, TX 76019 USA. RP Chen, AP (reprint author), Los Alamos Natl Lab, Ctr Integrated Nanotechnol CINT, POB 1663, Los Alamos, NM 87545 USA. EM qxjia@lanl.gov RI Chen, Aiping/F-3212-2011 OI Chen, Aiping/0000-0003-2639-2797 FU NNSA's Laboratory Directed Research and Development Program; U.S. DOD/ARO [W911NF-11-1-0507]; Center for Nanostructured Materials and Characterization Center for Materials and Biology at the University of Texas at Arlington FX The work has been supported by the NNSA's Laboratory Directed Research and Development Program and was performed, in part, at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science. The work at the University of Texas at Arlington has been supported by the U.S. DOD/ARO under Grant No. W911NF-11-1-0507, and the Center for Nanostructured Materials and Characterization Center for Materials and Biology at the University of Texas at Arlington. NR 18 TC 2 Z9 2 U1 4 U2 41 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAR 16 PY 2015 VL 106 IS 11 AR 111907 DI 10.1063/1.4915504 PG 4 WC Physics, Applied SC Physics GA CE1TS UT WOS:000351595500022 ER PT J AU Castelle, CJ Wrighton, KC Thomas, BC Hug, LA Brown, CT Wilkins, MJ Frischkorn, KR Tringe, SG Singh, A Markillie, LM Taylor, RC Williams, KH Banfield, JF AF Castelle, Cindy J. Wrighton, Kelly C. Thomas, Brian C. Hug, Laura A. Brown, Christopher T. Wilkins, Michael J. Frischkorn, Kyle R. Tringe, Susannah G. Singh, Andrea Markillie, Lye Meng Taylor, Ronald C. Williams, Kenneth H. Banfield, Jillian F. TI Genomic Expansion of Domain Archaea Highlights Roles for Organisms from New Phyla in Anaerobic Carbon Cycling SO CURRENT BIOLOGY LA English DT Article ID PYROCOCCUS-FURIOSUS; METABOLISM; INSIGHTS; DIVERSITY; EVOLUTION; SEDIMENTS; PATHWAY; ENVIRONMENTS; COMMUNITIES; MEMBRANE AB Background: Archaea represent a significant fraction of Earth's biodiversity, yet they remain much less well understood than Bacteria. Gene surveys, a few metagenomic studies, and some single-cell sequencing projects have revealed numerous little-studied archaeal phyla. Certain lineages appear to branch deeply and may be part of a major phylum radiation. The structure of this radiation and the physiology of the organisms remain almost unknown. Results: We used genome-resolved metagenomic analyses to investigate the diversity, genomes sizes, metabolic capacities, and potential roles of Archaea in terrestrial subsurface biogeochemical cycles. We sequenced DNA from complex sediment and planktonic consortia from an aquifer adjacent to the Colorado River (USA) and reconstructed the first complete genomes for Archaea using cultivation-independent methods. To provide taxonomic context, we analyzed an additional 151 newly sampled archaeal sequences. We resolved two new phyla within a major, apparently deep-branching group of phyla (a superphylum). The organisms have small genomes, and metabolic predictions indicate that their primary contributions to Earth's biogeochemical cycles involve carbon and hydrogen metabolism, probably associated with symbiotic and/or fermentation-based lifestyles. Conclusions: The results dramatically expand genomic sampling of the domain Archaea and clarify taxonomic designations within a major superphylum. This study, in combination with recently published work on bacterial phyla lacking cultivated representatives, reveals a fascinating phenomenon of major radiations of organisms with small genomes, novel proteome composition, and strong interdependence in both domains. C1 [Castelle, Cindy J.; Thomas, Brian C.; Hug, Laura A.; Singh, Andrea; Banfield, Jillian F.] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. [Wrighton, Kelly C.; Wilkins, Michael J.] Ohio State Univ, Dept Microbiol, Columbus, OH 43210 USA. [Brown, Christopher T.] Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. [Wilkins, Michael J.] Ohio State Univ, Sch Earth Sci, Columbus, OH 43210 USA. [Frischkorn, Kyle R.] Columbia Univ, Dept Earth & Environm Sci, New York, NY 10964 USA. [Frischkorn, Kyle R.] Columbia Univ, Lamont Doherty Earth Observ, New York, NY 10964 USA. [Tringe, Susannah G.] DOE Joint Genome Inst, Metagenome Program, Walnut Creek, CA 94598 USA. [Markillie, Lye Meng; Taylor, Ronald C.] Pacific NW Natl Lab, Div Biol Sci, Environm Mol Sci Lab, Richland, WA 99352 USA. [Williams, Kenneth H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Banfield, Jillian F.] Univ Calif Berkeley, Dept Environm Sci Policy & Management, Berkeley, CA 94720 USA. RP Banfield, JF (reprint author), Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. EM jbanfield@berkeley.edu RI Williams, Kenneth/O-5181-2014; Wilkins, Michael/A-9358-2013; OI Williams, Kenneth/0000-0002-3568-1155; Tringe, Susannah/0000-0001-6479-8427; Taylor, Ronald/0000-0001-9777-9767 FU US Department of Energy (DOE), Office of Science, Office of Biological and Environmental Research [DE-AC02-05CH11231, DE-SC0004918]; US DOE Joint Genome Institute, a DOE Office of Science User Facility [DE-AC02-05CH11231]; DOE Office of Biological and Environmental Research; US DOE [AC06-76RLO 1830]; Natural Sciences and Engineering Research Council of Canada FX This research was supported by the US Department of Energy (DOE), Office of Science, Office of Biological and Environmental Research under award number DE-AC02-05CH11231 (Sustainable Systems Scientific Focus Area; Lawrence Berkley National Laboratory operated by the University of California) and award number DE-SC0004918 (Systems Biology Knowledge Base Focus Area). Sequencing was performed at the US DOE Joint Genome Institute, a DOE Office of Science User Facility, supported under contract DE-AC02-05CH11231. Transcriptomics work was conducted at the Environmental Molecular Sciences Laboratory, a National Scientific User Facility sponsored by the DOE Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory (PNNL). PNNL is operated by Battelle for the US DOE under contract AC06-76RLO 1830. L.A.H. was partially supported by a Natural Sciences and Engineering Research Council of Canada postdoctoral fellowship. NR 59 TC 58 Z9 58 U1 8 U2 51 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0960-9822 EI 1879-0445 J9 CURR BIOL JI Curr. Biol. PD MAR 16 PY 2015 VL 25 IS 6 BP 690 EP 701 DI 10.1016/j.cub.2015.01.014 PG 12 WC Biochemistry & Molecular Biology; Cell Biology SC Biochemistry & Molecular Biology; Cell Biology GA CD7YN UT WOS:000351312100018 PM 25702576 ER PT J AU Iturrondobeitia, A Goni, A de Muro, IG Lezama, L Kim, C Doeff, M Cabana, J Rojo, T AF Iturrondobeitia, Amaia Goni, Aintzane Gil de Muro, Izaskun Lezama, Luis Kim, Chunjoong Doeff, Marca Cabana, Jordi Rojo, Teofilo TI High-Voltage Cathode Materials for Lithium-Ion Batteries: Freeze-Dried LiMn0.8Fe0.1M0.1PO4/C (M = Fe, Co, Ni, Cu) Nanocomposites SO INORGANIC CHEMISTRY LA English DT Article ID ENHANCED ELECTROCHEMICAL PERFORMANCE; MANGANESE PHOSPHATE; LIMNPO4 CATHODE; CATION SUBSTITUTION; LIFEPO4; SIZE; COMPOSITES; SI(IV) AB Four LiMn0.8Fe0.1M0.1PO4/C (M = Fe, Co, Ni, Cu) cathode materials have been synthesized via a freeze-drying method. The samples have been characterized by powder X-ray diffraction, transmission electron microscopy, magnetic susceptibility, and electrochemical measurements. The composition and effective insertion of the transition-metal substituents in LiMnPO4 have been corroborated by elemental analysis, the evolution of the crystallographic parameters, and the magnetic properties. The morphological characterization of the composites has demonstrated that the phosphate nanoparticles are enclosed in a matrix of amorphous carbon. Among them, LiMn0.8Fe0.1Ni0.1PO4/C is the most promising cathode material, providing a good electrochemical performance in all aspects: high voltage and specific capacity values, excellent cyclability, and good rate capability. This result has been attributed to several factors, such as the suitable morphology of the sample, the good connection afforded by the in situ generated carbon, and the amelioration of the structural stress provided by the presence of Ni2+ and Fe2+ in the olivine structure. C1 [Iturrondobeitia, Amaia; Goni, Aintzane; Gil de Muro, Izaskun; Lezama, Luis; Rojo, Teofilo] UPV, EHU, Dept Quim Inorgan, Bilbao 48080, Spain. [Iturrondobeitia, Amaia; Rojo, Teofilo] CIC EnergiGUNE, Minano 01510, Alava, Spain. [Goni, Aintzane; Gil de Muro, Izaskun; Lezama, Luis] BCMaterials, Derio 48160, Spain. [Kim, Chunjoong; Cabana, Jordi] Univ Illinois, Dept Chem, Chicago, IL 60607 USA. [Doeff, Marca] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. RP Rojo, T (reprint author), UPV, EHU, Dept Quim Inorgan, POB 644, Bilbao 48080, Spain. EM trojo@cicenergigune.com RI Rojo, Teofilo/B-5197-2015; Cabana, Jordi/G-6548-2012; IZASKUN, GIL DE MURO/F-3733-2016; Lezama, Luis/M-1544-2013; OI Rojo, Teofilo/0000-0003-2711-8458; Cabana, Jordi/0000-0002-2353-5986; Lezama, Luis/0000-0001-6183-2052; Goni, Aintzane/0000-0001-6914-5943 FU Ministerio de Educacion y Ciencia [MAT2013-41128-R]; Universidad del Pais Vasco/Euskal Herriko Unibertsitatea; Gobierno Vasco/Eusko Jaurlaritza [IT570-13]; Gobierno Vasco/Eusko Jaurlaritza (Etortek CIC EnergiGUNE 10); Gobierno Vasco/Eusko Jaurlaritza; Office of Vehicle Technologies, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was financially supported by the Ministerio de Educacion y Ciencia (Grant MAT2013-41128-R), the Universidad del Pais Vasco/Euskal Herriko Unibertsitatea, and the Gobierno Vasco/Eusko Jaurlaritza (IT570-13, Etortek CIC EnergiGUNE 10). A.I. thanks the Gobierno Vasco/Eusko Jaurlaritza for a fellowship. Portions of this work were supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies, of the U.S. Department of Energy under Contract DE-AC02-05CH11231 under the Batteries for Advanced Transportation Technologies (BATT) Program. NR 48 TC 4 Z9 4 U1 8 U2 100 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD MAR 16 PY 2015 VL 54 IS 6 BP 2671 EP 2678 DI 10.1021/ic5028306 PG 8 WC Chemistry, Inorganic & Nuclear SC Chemistry GA CD8DK UT WOS:000351325200021 PM 25723381 ER PT J AU Hasegawa, G Sato, T Kanamori, K Sun, CJ Ren, Y Kobayashi, Y Kageyama, H Abe, T Nakanishi, K AF Hasegawa, George Sato, Tatsuya Kanamori, Kazuyoshi Sun, Cheng-Jun Ren, Yang Kobayashi, Yoji Kageyama, Hiroshi Abe, Takeshi Nakanishi, Kazuki TI Effect of Calcination Conditions on Porous Reduced Titanium Oxides and Oxynitrides via a Preceramic Polymer Route SO INORGANIC CHEMISTRY LA English DT Article ID CARBOTHERMAL SYNTHESIS; THIN-FILMS; TIO2; TIN; REDUCTION; NITRIDE; SYSTEM; OXYGEN; SPECTROSCOPY; TRANSITIONS AB A preceramic polymer route from Ti-based inorganicorganic hybrid networks provides electroconductive N-doped reduced titanium oxides (Ti(n)O2(n-1)) and titanium oxynitrides (TiOxNy) with a monolithic shape as well as well-defined porous structures. This methodology demonstrates an advantageously lower temperature of the crystal phase transition compared to the reduction of TiO2 by carbon or hydrogen. In this study, the effect of calcination conditions on various features of the products has been explored by adopting three different atmospheric conditions and varying the calcination temperature. The detailed crystallographic and elemental analyses disclose the distinguished difference in the phase transition behavior with respect to the calcination atmosphere. The correlation between the crystallization and nitridation behaviors, porous properties, and electric conductivities in the final products is discussed. C1 [Hasegawa, George; Kobayashi, Yoji; Kageyama, Hiroshi; Abe, Takeshi] Kyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, Japan. [Sato, Tatsuya; Kanamori, Kazuyoshi; Nakanishi, Kazuki] Kyoto Univ, Grad Sch Sci, Dept Chem, Sakyo Ku, Kyoto 6068502, Japan. [Sun, Cheng-Jun; Ren, Yang] Argonne Natl Lab, APS, Xray Sci Div, Argonne, IL 60439 USA. [Kageyama, Hiroshi] Japan Sci & Technol Agcy, CREST, Kawaguchi, Saitama 3320012, Japan. RP Hasegawa, G (reprint author), Kyoto Univ, Grad Sch Engn, Dept Energy & Hydrocarbon Chem, Nishikyo Ku, Kyoto 6158510, Japan. EM h-george@elech.kuic.kyoto-u.ac.jp RI Hasegawa, George/A-1653-2014; Abe, Takeshi/F-2544-2010; Kageyama, Hiroshi/A-4602-2010; Nakanishi, Kazuki/A-1814-2012; Kanamori, Kazuyoshi/A-5561-2011 OI Hasegawa, George/0000-0003-4546-5197; Kanamori, Kazuyoshi/0000-0001-5087-9808 FU Japan Society for the Promotion of Science (JSPS) [24.31]; U.S. Department of Energy (DOE), Basic Energy Sciences; Canadian Light Source; University of Washington; APS; U.S. DOE [DE-AC02-06CH11357] FX The present work was supported by a Grant-in-Aid for JSPS Fellows (Grant 24.31 to G.H.) from the Japan Society for the Promotion of Science (JSPS). PNC/XSD facilities at the APS and research at these facilities are supported by the U.S. Department of Energy (DOE), Basic Energy Sciences, the Canadian Light Source and its funding partners, the University of Washington, and the APS. Use of the APS, an Office of Science User Facility, operated for the U.S. DOE, Office of Science, by Argonne National Laboratory was supported by the U.S. DOE under Contract DE-AC02-06CH11357. NR 45 TC 2 Z9 2 U1 5 U2 31 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD MAR 16 PY 2015 VL 54 IS 6 BP 2802 EP 2808 DI 10.1021/ic502972v PG 7 WC Chemistry, Inorganic & Nuclear SC Chemistry GA CD8DK UT WOS:000351325200034 PM 25731074 ER PT J AU Bogart, JA Lewis, AJ Boreen, MA Lee, HB Medling, SA Carroll, PJ Booth, CH Schelter, EJ AF Bogart, Justin A. Lewis, Andrew J. Boreen, Michael A. Lee, Heui Beom Medling, Scott A. Carroll, Patrick J. Booth, Corwin H. Schelter, Eric J. TI A Ligand Field Series for the 4f-Block from Experimental and DFT Computed Ce(IV/III) Electrochemical Potentials SO INORGANIC CHEMISTRY LA English DT Article ID REDUCTION POTENTIALS; CERIUM(IV) COMPLEXES; AMMONIUM-NITRATE; WATER OXIDATION; LANTHANIDE; CEROCENE; RESONANCE; CRYSTAL; OXIDANT; STATE AB Understanding of the sensitivity of the red-action potential of Cerium(IV) cations to ligand field, strength has yet to benefit from systematic variation of the ligand environment. Detailed analyses for a series of seven cerium(W) tetralds(pyridyl-nitroxide) compounds and their cerium(III) analogues in varying ligand field Strengths are presented. Electrochemical, spectroscopic, and computational results reveal a dose correlation of electronic properties with ligand substituents. Together with electrochernical data for reported eight-coordinate compounds, DET calculations reveal a broad range of the cerium(IV/III) redox potentials correlated to ligand field strengths, establishing a semiempirical, predictive model for the modulation of cerium redox thermodynamics and ligand field strengths. Applications over a variety of scientific disciplines make use of the fundamental redox thermodynamics of cerium. Such applications will benefit from a combined experimental and theoretical approach for assessing redox cycling of cerium compounds. C1 [Bogart, Justin A.; Lewis, Andrew J.; Boreen, Michael A.; Lee, Heui Beom; Carroll, Patrick J.; Schelter, Eric J.] Univ Penn, Dept Chem, P Roy & Diana T Vagelos Labs, Philadelphia, PA 19104 USA. [Medling, Scott A.; Booth, Corwin H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Schelter, EJ (reprint author), Univ Penn, Dept Chem, P Roy & Diana T Vagelos Labs, Philadelphia, PA 19104 USA. EM schelter@sas.upenn.edu FU U.S. Department of Energy, Office of Science, Early Career Research Program [DE-SC0006518]; Research Corporation for Science Advancement; University of Pennsylvania; National Science Foundation [OCI-1053575]; Office of Science (OS), Office of Basic Energy Sciences, of the U.S. Department of Energy (DOE) [DE-AC02-05CH11231] FX E.J.S. acknowledges the U.S. Department of Energy, Office of Science, Early Career Research Program (Grant DE-SC0006518), the Research Corporation for Science Advancement (Cottrell Scholar Award to E.J.S.), and the University of Pennsylvania for financial support of this work. This work used the Extreme Science and Engineering Discovery Environment (XSEDE), which is supported by the National Science Foundation Grant OCI-1053575. Portions of this work were supported by the Director, Office of Science (OS), Office of Basic Energy Sciences, of the U.S. Department of Energy (DOE) under Contract No. DE-AC02-05CH11231 and were carried out at SSRL, a Directorate of SLAC National Accelerator Laboratory and an OS user facility operated for the DOE OS by Stanford University. NR 45 TC 13 Z9 13 U1 4 U2 37 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD MAR 16 PY 2015 VL 54 IS 6 BP 2830 EP 2837 DI 10.1021/ic503000z PG 8 WC Chemistry, Inorganic & Nuclear SC Chemistry GA CD8DK UT WOS:000351325200037 PM 25710199 ER PT J AU Gonzalez, MI Bloch, ED Mason, JA Teat, SJ Long, JR AF Gonzalez, Miguel I. Bloch, Eric D. Mason, Jarad A. Teat, Simon J. Long, Jeffrey R. TI Single-Crystal-to-Single-Crystal Metalation of a Metal-Organic Framework: A Route toward Structurally Well-Defined Catalysts SO INORGANIC CHEMISTRY LA English DT Article ID C-H BORYLATION; HETEROGENEOUS CATALYSTS; ASYMMETRIC CATALYSIS; MOLECULAR-STRUCTURES; COMPLEXES; SITES; OXIDATION; LIGAND; FUNCTIONALIZATION; CHEMISTRY AB Metal organic frameworks featuring ligands with open chelating groups are versatile platforms for the preparation of a diverse set of heterogeneous catalysts through postsynthetic metalation. The crystalline nature of these materials allows them to be characterized via X-ray diffraction, which provides valuable insight into the structure of the metal sites that facilitate catalysis. A highly porous and thermally robust zirconium-based metal organic framework, Zr6O4(OH)(4)(bpydc)(6)(bpydc(2-) = 2,2'-bipyridne-5,5'-dicarboxylate), bears open bipyridine sites that readily react with a variety of solution- and gas-phase metal sources to form the corresponding metalated frameworks. Remarkably, Zr6O4(OH)(4)(bpydc)(6) undergoes a single-crystal-to-single-crystal transformation upon metalation that involves a change in space group from Fm (3) over barm to Pa (3) over bar. This structural transformation leads to an ordering of the metalated linkers within the framework, allowing structural characterization of the resulting metal complexes. Furthermore, Zr6O4(OH)(4)(bpydc)(6) yields an active heterogeneous catalyst for arene C-H borylation when metalated with [Ir(COD)(2)]BF4 (COD = 1,5-cyclooctadiene). These results highlight the unique potential of metal-organic frameworks as a class of heterogeneous catalysts that allow unparalleled structural characterization and control over their active sites. C1 [Gonzalez, Miguel I.; Bloch, Eric D.; Mason, Jarad A.; Long, Jeffrey R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Teat, Simon J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Long, Jeffrey R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Long, JR (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM jrlong@berkeley.edu OI Gonzalez, Miguel/0000-0003-4250-9035 FU Laboratory Directed Research and Development Program of Lawrence Berkeley National Laboratory under U.S. Department of Energy [DE-AC02-05CH11231]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; Gerald K. Branch; Arkema; Chevron FX This work was supported by the Laboratory Directed Research and Development Program of Lawrence Berkeley National Laboratory under U.S. Department of Energy Contract DE-AC02-05CH11231. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract DE-AC02-05CH11231. We thank the 11-BM staff at the Advanced Photon Source at Argonne National Laboratory for assisting with powder X-ray diffraction experiments. Use of the Advanced Photon Source at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract DE-AC02-06CH11357. We thank Gerald K. Branch and Arkema for the fellowship support of E.D.B and Chevron for fellowship support of J.A.M. We are grateful for the assistance of Antonio DiPasquale and Kevin J. Gagnon with single-crystal X-ray diffraction experiments and Jonathan Bachman with SEM measurements. We also thank Kohei Takahashi, Matthew Larsen, and Carl Liskey for fruitful discussions. NR 68 TC 35 Z9 35 U1 8 U2 63 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD MAR 16 PY 2015 VL 54 IS 6 BP 2995 EP 3005 DI 10.1021/acs.inorgchem.5b00096 PG 11 WC Chemistry, Inorganic & Nuclear SC Chemistry GA CD8DK UT WOS:000351325200055 PM 25719803 ER PT J AU Van Allsburg, KM Anzenberg, E Drisdell, WS Yano, J Tilley, TD AF Van Allsburg, Kurt M. Anzenberg, Eitan Drisdell, Walter S. Yano, Junko Tilley, T. Don TI Oxygen-Atom Transfer Chemistry and Thermolytic Properties of a Di-tert-Butylphosphate-Ligated Mn4O4 Cubane SO CHEMISTRY-A EUROPEAN JOURNAL LA English DT Article DE artificial photosynthesis; cubanes; oxygen-atom transfer; thermolytic molecular precursor; water oxidation ID PHOTOSYNTHETIC WATER OXIDATION; DOUBLE-PIVOT MECHANISM; PHOTOSYSTEM-II; MOLECULAR PRECURSOR; CATALYTIC-OXIDATION; DI(TERT-BUTYL)PHOSPHATE COMPLEXES; EPOXIDATION CATALYSTS; MULTICOMPONENT OXIDES; MANGANESE COMPLEXES; CRYSTAL-STRUCTURES AB [Mn4O4{O2P(OtBu)(2)}(6)] (1), an Mn4O4 cubane complex combining the structural inspiration of the photosystem II oxygen-evolving complex with thermolytic precursor ligands, was synthesized and fully characterized. Core oxygen atoms within complex 1 are transferred upon reaction with an oxygen-atom acceptor (PEt3), to give the butterfly complex [Mn4O2{O2P(OtBu)(2)}(6)(OPEt3)(2)]. The cubane structure is restored by reaction of the latter complex with the O-atom donor PhIO. Complex 1 was investigated as a precursor to inorganic Mn metaphosphate/pyrophosphate materials, which were studied by X-ray absorption spectroscopy to determine the fate of the Mn4O4 unit. Under the conditions employed, thermolyses of 1 result in reduction of the manganese to Mn-II species. Finally, the related butterfly complex [Mn4O2{O2P(pin)}(6)(bpy)(2)] (pin=pinacolate) is described. C1 [Van Allsburg, Kurt M.; Tilley, T. Don] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Van Allsburg, Kurt M.; Anzenberg, Eitan; Drisdell, Walter S.; Yano, Junko; Tilley, T. Don] Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA USA. [Van Allsburg, Kurt M.; Anzenberg, Eitan; Drisdell, Walter S.] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA USA. [Yano, Junko] Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA USA. [Tilley, T. Don] Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA USA. RP Tilley, TD (reprint author), Univ Calif Berkeley, Dept Chem, 420 Latimer Hall, Berkeley, CA 94720 USA. EM tdtilley@berkeley.edu FU Office of Science of the U.S. Department of Energy [DE-SC0004993]; National Science Foundation Graduate Research Fellowship [DGE-1106400]; NIH Shared Instrumentation Grant [S10RR027172]; Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231] FX J. M. Zadrozny and J. R. Long (magnetic susceptibility), A. T. Iavarone (ESI-TOF-MS), M. S. Ziegler (single-crystal XRD), and W. Kim and H. Frei (MS detection of O2) are gratefully acknowledged for their contributions in characterizing the compounds herein. This material is based upon work performed by the Joint Center for Artificial Photosynthesis, a DOE Energy Innovation Hub, supported through the Office of Science of the U.S. Department of Energy under Award Number DE-SC0004993. K.M.V. acknowledges support from a National Science Foundation Graduate Research Fellowship under Grant No. DGE-1106400. Single-crystal X-ray structure determination was supported by NIH Shared Instrumentation Grant S10RR027172. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 72 TC 2 Z9 2 U1 2 U2 21 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 0947-6539 EI 1521-3765 J9 CHEM-EUR J JI Chem.-Eur. J. PD MAR 16 PY 2015 VL 21 IS 12 BP 4646 EP 4654 DI 10.1002/chem.201406114 PG 9 WC Chemistry, Multidisciplinary SC Chemistry GA CD0KA UT WOS:000350760000026 PM 25676196 ER PT J AU Wang, JJA Ren, F Tan, T Liu, K AF Wang, John Jy-An Ren, Fei Tan, Ting Liu, Ken TI The development of in situ fracture toughness evaluation techniques in hydrogen environment (vol 40, pg 2013, 2015) SO INTERNATIONAL JOURNAL OF HYDROGEN ENERGY LA English DT Correction C1 [Wang, John Jy-An; Ren, Fei; Tan, Ting; Liu, Ken] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Wang, JJA (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. EM wangja@ornl.gov OI Wang, Jy-An/0000-0003-2402-3832 NR 1 TC 0 Z9 0 U1 0 U2 1 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-3199 EI 1879-3487 J9 INT J HYDROGEN ENERG JI Int. J. Hydrog. Energy PD MAR 16 PY 2015 VL 40 IS 10 BP 4034 EP 4034 DI 10.1016/j.ijhydene.2015.01.082 PG 1 WC Chemistry, Physical; Electrochemistry; Energy & Fuels SC Chemistry; Electrochemistry; Energy & Fuels GA CD2WO UT WOS:000350939900024 ER PT J AU Campione, S Brener, I Marquier, F AF Campione, Salvatore Brener, Igal Marquier, Francois TI Theory of epsilon-near-zero modes in ultrathin films SO PHYSICAL REVIEW B LA English DT Article ID THIN METAL-FILMS; OPTICAL-PROPERTIES; SURFACE-PLASMONS; ABSORPTION; EMISSION; WAVES AB The physics of the epsilon-near-zero (ENZ) mode, which is supported by a nanolayer at the frequency where the dielectric permittivity vanishes, has recently been a subject of debate. In this Rapid Communication, we thoroughly investigate and clarify the physics of this mode, providing its main characteristics and its domain of existence. This understanding will benefit all the applications that rely on ENZ modes in semiconductor nanolayers, including directional perfect absorption, voltage-tunable devices, and ultrafast thermal emission. C1 [Campione, Salvatore; Brener, Igal] Sandia Natl Labs, Ctr Integrated Nanotechnol CINT, Albuquerque, NM 87185 USA. [Campione, Salvatore; Brener, Igal] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Marquier, Francois] Univ Paris Sud, CNRS, Inst Opt, Lab Charles Fabry, F-91127 Palaiseau, France. RP Campione, S (reprint author), Sandia Natl Labs, Ctr Integrated Nanotechnol CINT, POB 5800, Albuquerque, NM 87185 USA. EM sncampi@sandia.gov; francois.marquier@institutoptique.fr RI Marquier, Francois/A-2359-2015 OI Marquier, Francois/0000-0003-3118-1150 FU French Ministry of Defense through ERE Grant from the Direction Generale de l'Armement (DGA) [2014.60.0082]; US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; US Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; Lockheed Martin Corporation FX F.M. acknowledges financial support from the French Ministry of Defense through ERE Grant No. 2014.60.0082 from the Direction Generale de l'Armement (DGA). This work was supported by the US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. It was performed, in part, at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the US Department of Energy (DOE) Office of Science. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the US Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 31 TC 15 Z9 15 U1 5 U2 37 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAR 16 PY 2015 VL 91 IS 12 AR 121408 DI 10.1103/PhysRevB.91.121408 PG 5 WC Physics, Condensed Matter SC Physics GA CD4FQ UT WOS:000351038400005 ER PT J AU Cao, C Tao, R Ford, DC Klie, RF Proslier, T Cooley, LD Dzyuba, A Zapol, P Warren, M Lind, H Zasadzinski, JF AF Cao, C. Tao, R. Ford, D. C. Klie, R. F. Proslier, T. Cooley, L. D. Dzyuba, A. Zapol, P. Warren, M. Lind, H. Zasadzinski, J. F. TI Giant two-phonon Raman scattering from nanoscale NbC precipitates in Nb SO PHYSICAL REVIEW B LA English DT Article ID TRANSITION-METALS; SUPERCONDUCTOR; TEMPERATURE; NIOBIUM AB High-purity niobium (Nb), subjected to the processing methods used in the fabrication of superconducting rf cavities, displays micrometer-sized surface patches containing excess carbon. High-resolution transmission electron microscopy and electron energy-loss spectroscopy measurements are presented which reveal the presence of nanoscale NbC coherent precipitates in such regions. Raman backscatter spectroscopy on similar surface regions exhibit spectra consistent with the literature results on bulk NbC but with significantly enhanced two-phonon scattering. The unprecedented strength and sharpness of the two-phonon signal has prompted a theoretical analysis, using density functional theory (DFT), of phonon modes in NbC for two different interface models of the coherent precipitate. One model leads to overall compressive strain and a comparison to ab initio calculations of phonon dispersion curves under uniform compression of the NbC shows that the measured two-phonon peaks are linked directly to phonon anomalies arising from strong electron-phonon interaction. Another model of the extended interface between Nb and NbC, studied by DFT, gives insight into the frequency shifts of the acoustic and optical mode density of states measured by first-order Raman spectroscopy. The exact origin of the stronger two-phonon response is not known at present but it suggests the possibility of enhanced electron-phonon coupling in transition-metal carbides under strain found either in the bulk NbC inclusions or at their interfaces with Nb metal. Preliminary tunneling studies using a point contact method show some energy gaps larger than expected for bulk NbC. C1 [Cao, C.; Warren, M.; Zasadzinski, J. F.] IIT, Dept Phys, Chicago, IL 60616 USA. [Cao, C.; Ford, D. C.; Proslier, T.; Zapol, P.; Zasadzinski, J. F.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Tao, R.; Klie, R. F.] Univ Illinois, Dept Phys, Chicago, IL 60607 USA. [Cooley, L. D.; Dzyuba, A.] Fermilab Natl Accelerator Lab, Tech Div, Superconducting Mat Dept, Batavia, IL 60510 USA. [Lind, H.] Linkoping Univ, Dept Phys Chem & Biol IFM, SE-58183 Linkoping, Sweden. RP Zasadzinski, JF (reprint author), IIT, Dept Phys, Chicago, IL 60616 USA. EM zasadzinski@iit.edu RI Cooley, Lance/E-7377-2015; Zapol, Peter/G-1810-2012 OI Cooley, Lance/0000-0003-3488-2980; Zapol, Peter/0000-0003-0570-9169 FU SSF; Swedish Research Council; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; Department of Energy, Office of Science, Office of High Energy Physics [50335] FX The authors thank G. Ciovati of Jefferson Laboratory for supplying Nb samples used in this study. Calculations (H.L.) were performed with financial support by the SSF-project Designed multicomponent coatings, MultiFilms and the Swedish Research Council. Calculations were carried out at the Swedish National Infrastructure for Computing (SNIC), Argonne LCRC and Argonne Center for Nanoscale Materials. The work at Argonne National Laboratory and the use of the Center for Nanoscale Materials and the Electron Microscopy center at Argonne National Laboratory were supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Contract No. DE-AC02-06CH11357. This work was also supported by the Department of Energy, Office of Science, Office of High Energy Physics, early career award FWP#50335 to T.P. NR 37 TC 4 Z9 4 U1 2 U2 25 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAR 16 PY 2015 VL 91 IS 9 AR 094302 DI 10.1103/PhysRevB.91.094302 PG 9 WC Physics, Condensed Matter SC Physics GA CD4FB UT WOS:000351036900002 ER PT J AU Karrasch, C Kennes, DM Heidrich-Meisner, F AF Karrasch, C. Kennes, D. M. Heidrich-Meisner, F. TI Spin and thermal conductivity of quantum spin chains and ladders SO PHYSICAL REVIEW B LA English DT Article ID DENSITY-MATRIX RENORMALIZATION; XXZ CHAIN; HEISENBERG-MODEL; PRODUCT STATES; TRANSPORT; SYSTEMS; TEMPERATURE; DYNAMICS; EXCITATIONS; LIQUID AB We study the spin and thermal conductivity of spin-1/2 ladders and chains at finite temperature, relevant for experiments with quantum magnets. Using a state-of-the-art density matrix renormalization group algorithm, we compute the current autocorrelation functions on the real-time axis and then carry out a Fourier integral to extract the frequency dependence of the corresponding conductivities. The finite-time error is analyzed carefully. We first investigate the limiting case of spin-1/2 XXZ chains, for which our analysis suggests nonzero dc conductivities in all interacting cases irrespective of the presence or absence of spin Drude weights. For ladders, we observe that all models studied are normal conductors with no ballistic contribution. Nonetheless, only the high-temperature spin conductivity of XX ladders has a simple diffusive, Drude-like form, while Heisenberg ladders exhibit a more complicated low-frequency behavior. We compute the dc spin conductivity down to temperatures of the order of T similar to 0.5J, where J is the exchange coupling along the legs of the ladder. We further extract mean-free paths and discuss our results in relation to thermal conductivity measurements on quantum magnets. C1 [Karrasch, C.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 95720 USA. [Karrasch, C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Kennes, D. M.] Rhein Westfal TH Aachen, Inst Theorie Stat Phys, D-52056 Aachen, Germany. [Kennes, D. M.] JARA Fundamentals Future Informat Technol, D-52056 Aachen, Germany. [Heidrich-Meisner, F.] Univ Munich, Dept Phys, D-80333 Munich, Germany. [Heidrich-Meisner, F.] Univ Munich, Arnold Sommerfeld Ctr Theoret Phys, D-80333 Munich, Germany. RP Karrasch, C (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 95720 USA. RI Heidrich-Meisner, Fabian/B-6228-2009; Karrasch, Christoph/S-5716-2016 OI Karrasch, Christoph/0000-0002-6475-3584 FU Nanostructured Thermoelectrics program of LBNL; DFG through the Research Training Group [FOR 912, HE-5242/2-2] FX We thank W. Brenig, P. Prelovsek, T. Prosen, R. Steinigeweg, and X. Zotos for very useful discussions. We are further indebted to X. Zotos for sending us exact-diagonalization data from Ref. [75] and Bethe-ansatz results for Ds(T) computed with the methods of Ref. [38] for comparison. We acknowledge support by the Nanostructured Thermoelectrics program of LBNL (C.K.) as well as by the DFG through the Research Training Group 1995 (D.M.K) and through FOR 912 via Grant No. HE-5242/2-2 (F.H.-M.). NR 119 TC 11 Z9 11 U1 1 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAR 16 PY 2015 VL 91 IS 11 AR 115130 DI 10.1103/PhysRevB.91.115130 PG 10 WC Physics, Condensed Matter SC Physics GA CD4FG UT WOS:000351037400002 ER PT J AU Lucy, JM Hauser, AJ Liu, Y Zhou, H Choi, Y Haskel, D te Velthuis, SGE Yang, FY AF Lucy, J. M. Hauser, A. J. Liu, Y. Zhou, H. Choi, Y. Haskel, D. te Velthuis, S. G. E. Yang, F. Y. TI Depth-resolved magnetic and structural analysis of relaxing epitaxial Sr2CrReO6 SO PHYSICAL REVIEW B LA English DT Article ID CIRCULAR-DICHROISM AB Structural relaxation in a Sr2CrReO6 epitaxial film, which exhibits strong spin-orbit coupling, leads to depth-dependent magnetism. We combine two depth-resolved synchrotron x-ray techniques-two-dimensional reciprocal space mapping and x-ray magnetic circular dichroism-to quantitatively determine this effect. An 800-nm-thick film of Sr2CrReO6, grown with tensile epitaxial strain on SrCr0.5Nb0.5O3(225 nm)/(LaAlO3)(0.3)(Sr2AlTaO6)(0.7), relaxes away from the Sr2CrReO6/SrCr0.5Nb0.5O3 interface to its bulk lattice parameters, with much of the film being fully relaxed. Grazing incidence x-ray diffraction of the film elucidates the in-plane strain relaxation near the film-substrate interface, while depth-resolved x-ray magnetic circular dichroism at the Re L edge reveals the magnetic contributions of the Re site. The smooth relaxation of the film near the interface correlates with changes in the magnetic anisotropy. This provides a systematic and powerful way to probe the depth-varying structural and magnetic properties of a complex oxide with synchrotron-source x-ray techniques. C1 [Lucy, J. M.; Yang, F. Y.] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. [Hauser, A. J.] Univ Calif Santa Barbara, California Nanosyst Inst, Santa Barbara, CA 93106 USA. [Liu, Y.; te Velthuis, S. G. E.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Zhou, H.; Choi, Y.; Haskel, D.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Lucy, JM (reprint author), Ohio State Univ, Dept Phys, 191 West Woodruff Ave, Columbus, OH 43210 USA. EM fyyang@physics.osu.edu RI Liu, Yaohua/B-2529-2009; te Velthuis, Suzanne/I-6735-2013 OI Liu, Yaohua/0000-0002-5867-5065; te Velthuis, Suzanne/0000-0002-1023-8384 FU Center for Emergent Materials at the Ohio State University, a National Science Foundation Materials Research Science and Engineering Center [DMR-1420451]; NanoSystems Laboratory; Center for Electron Microscopy and Analysis at the Ohio State University; Elings Prize Fellowship of the California Nanosystems Institute at the University of California, Santa Barbara; U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; DOE Office of Science by Argonne National Laboratory [DE-AC02-06CH11357] FX This work is supported by the Center for Emergent Materials at the Ohio State University, a National Science Foundation Materials Research Science and Engineering Center (Grant No. DMR-1420451). Partial support is provided by the NanoSystems Laboratory and the Center for Electron Microscopy and Analysis at the Ohio State University. A.J.H. acknowledges support through an Elings Prize Fellowship of the California Nanosystems Institute at the University of California, Santa Barbara. Work at MSD, ANL (Y.L. and S.t.V.) was supported by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. This research used resources (GIXD and XMCD) of the Advanced Photon Source, a U.S. DOE Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. NR 23 TC 1 Z9 1 U1 0 U2 19 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAR 16 PY 2015 VL 91 IS 9 AR 094413 DI 10.1103/PhysRevB.91.094413 PG 6 WC Physics, Condensed Matter SC Physics GA CD4FB UT WOS:000351036900004 ER PT J AU Urbanek, M Uhlir, V Lambert, CH Kan, JJ Eibagi, N Vanatka, M Flajsman, L Kalousek, R Im, MY Fischer, P Sikola, T Fullerton, EE AF Urbanek, Michal Uhlir, Vojtech Lambert, Charles-Henri Kan, Jimmy J. Eibagi, Nasim Vanatka, Marek Flajsman, Lukas Kalousek, Radek Im, Mi-Young Fischer, Peter Sikola, Tomas Fullerton, Eric E. TI Dynamics and efficiency of magnetic vortex circulation reversal SO PHYSICAL REVIEW B LA English DT Article ID STATE; PERMALLOY; DISKS; FIELD AB Dynamic switching of the vortex circulation in magnetic nanodisks by fast-rising magnetic field pulse requires annihilation of the vortex core at the disk boundary and reforming a new vortex with the opposite sense of circulation. Here we study the influence of pulse parameters on the dynamics and efficiency of the vortex core annihilation in permalloy (Ni80Fe20) nanodisks. We use magnetic transmission soft x-ray microscopy to experimentally determine a pulse rise time-pulse amplitude phase diagram for vortex circulation switching and investigate the time-resolved evolution of magnetization in different regions of the phase diagram. The experimental phase diagram is compared with an analytical model based on Thiele's equation describing high-amplitude vortex core motion in a parabolic potential. We find that the analytical model is in good agreement with experimental data for a wide range of disk geometries. From the analytical model and in accordance with our experimental finding we determine the geometrical condition for dynamic vortex core annihilation and pulse parameters needed for the most efficient and fastest circulation switching. The comparison of our experimental results with micromagnetic simulations shows that the micromagnetic simulations of "ideal" disks with diameters larger than similar to 250 nm overestimate nonlinearities in susceptibility and eigenfrequency. This overestimation leads to the core polarity switching near the disk boundary, which then in disagreement with experimental findings prevents the core annihilation and circulation switching. We modify the micromagnetic simulations by introducing the "boundary region" of reduced magnetization to simulate the experimentally determined susceptibility and in these modified micromagnetic simulations we are able to reproduce the experimentally observed dynamic vortex core annihilation and circulation switching. C1 [Urbanek, Michal; Uhlir, Vojtech; Kalousek, Radek; Sikola, Tomas] Brno Univ Technol, CEITEC BUT, Brno 61600, Czech Republic. [Urbanek, Michal; Vanatka, Marek; Flajsman, Lukas; Kalousek, Radek; Sikola, Tomas] Brno Univ Technol, Inst Phys Engn, Brno 61600, Czech Republic. [Uhlir, Vojtech; Lambert, Charles-Henri; Kan, Jimmy J.; Eibagi, Nasim; Fullerton, Eric E.] Univ Calif San Diego, Ctr Magnet Recording Res, La Jolla, CA 92093 USA. [Lambert, Charles-Henri] Univ Lorraine, Inst Jean Lamour, UMR CNRS 7198, F-54506 Vandoeuvre Les Nancy, France. [Im, Mi-Young; Fischer, Peter] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Ctr Xray Opt, Berkeley, CA 94720 USA. [Im, Mi-Young] Daegu Gyeongbuk Inst Sci & Technol, Dept Emerging Mat Sci, Daegu 711873, South Korea. [Fischer, Peter] Univ Calif Santa Cruz, Dept Phys, Santa Cruz, CA 94056 USA. RP Urbanek, M (reprint author), Brno Univ Technol, CEITEC BUT, Brno 61600, Czech Republic. EM urbanek@fme.vutbr.cz; vojtech.uhlir@uh.cz RI Fischer, Peter/A-3020-2010; Sikola, Tomas/D-9875-2012; Uhlir, Vojtech/E-6860-2011; Urbanek, Michal/E-1136-2012; Fullerton, Eric/H-8445-2013 OI Fischer, Peter/0000-0002-9824-9343; Urbanek, Michal/0000-0003-0072-2073; Fullerton, Eric/0000-0002-4725-9509 FU European Regional Development Fund (CEITEC) [CZ.1.05/1.1.00/02.0068]; Grant Agency of the Czech Republic [P102/12/P443]; EU Seventh Framework Programme [286154-SYLICA, 280566-UnivSEM]; US Department of Energy (DOE), Office of Basic Energy Sciences [DE-SC0003678]; Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the US Department of Energy [DE-AC02-05-CH11231]; Leading Foreign Research Institute Recruitment Program through the National Research Foundation of Korea (NRF) - Ministry of Education, Science, and Technology (MEST) [2012K1A4A3053565] FX The research at BUT was supported by the European Regional Development Fund (CEITEC; CZ.1.05/1.1.00/02.0068), by the Grant Agency of the Czech Republic (Project No. P102/12/P443), and by the EU Seventh Framework Programme (Contracts No. 286154-SYLICA and 280566-UnivSEM). The research at UCSD was supported by the research programs of the US Department of Energy (DOE), Office of Basic Energy Sciences (Award No. DE-SC0003678). The operation of the x-ray microscope was supported by the Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the US Department of Energy under Contract No. DE-AC02-05-CH11231. P.F. and M.Y.I. acknowledge support by the Leading Foreign Research Institute Recruitment Program (Grant No. 2012K1A4A3053565) through the National Research Foundation of Korea (NRF) funded by the Ministry of Education, Science, and Technology (MEST). NR 34 TC 3 Z9 3 U1 1 U2 33 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 16 PY 2015 VL 91 IS 9 AR 094415 DI 10.1103/PhysRevB.91.094415 PG 11 WC Physics, Condensed Matter SC Physics GA CD4FB UT WOS:000351036900006 ER PT J AU Linder, EV AF Linder, Eric V. TI Quintessence's last stand? SO PHYSICAL REVIEW D LA English DT Article ID NAMBU-GOLDSTONE BOSONS; SAMPLES AB Current cosmological data puts increasing pressure on models of dark energy in the freezing class, e.g. early dark energy or those with equation of state w substantially different from -1. We investigate to what extent data will distinguish the thawing class of quintessence from a cosmological constant. Since thawing dark energy deviates from w = -1 only at late times, we find that deviations 1 + w less than or similar to 0.1 are difficult to see even with next generation measurements; however, modest redshift drift data can improve the sensitivity by a factor of two. Furthermore, technical naturalness prefers specific thawing models. C1 [Linder, Eric V.] Univ Calif Berkeley, Berkeley Ctr Cosmol Phys, Berkeley, CA 94720 USA. [Linder, Eric V.] Univ Calif Berkeley, Berkeley Lab, Berkeley, CA 94720 USA. RP Linder, EV (reprint author), Univ Calif Berkeley, Berkeley Ctr Cosmol Phys, Berkeley, CA 94720 USA. FU DOE [DE-SC-0007867]; Office of Science, Office of High Energy Physics, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work has been supported by DOE Grant No. DE-SC-0007867 and the Director, Office of Science, Office of High Energy Physics, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 25 TC 5 Z9 5 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 16 PY 2015 VL 91 IS 6 AR 063006 DI 10.1103/PhysRevD.91.063006 PG 5 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CD4GV UT WOS:000351041600003 ER PT J AU Bennett, SP Ambaye, H Lee, H LeClair, P Mankey, GJ Lauter, V AF Bennett, S. P. Ambaye, H. Lee, H. LeClair, P. Mankey, G. J. Lauter, V. TI Direct Evidence of Anomalous Interfacial Magnetization in Metamagnetic Pd doped FeRh Thin Films SO SCIENTIFIC REPORTS LA English DT Article ID EXCHANGE SPRING FILMS; ROOM-TEMPERATURE; RECORDING MEDIA; IRON-RHODIUM; ALLOYS; MAGNETISM AB Palladium doped iron rhodium is a magnetic material of significant interest for it's close to room temperature magnetostructural phase transition from antiferromagnetic (AF) to ferromagnetic (FM) ordering. Here we report on the peculiarities of the magnetization distribution in thin films of FeRh(Pd) probed by Polarized Neutron Reflectometry. Remarkably, we've found thin interfacial regions with strong magnetization that have unique thermomagnetic properties as compared to the rest of the system. These regions exist at the top and bottom interfaces of the films while the central regions behave similarly to the bulk with a clear AF-FM order transition. Further we explore the impact of an additional Pt interlayer introduced in the middle of the FeRh(Pd) film and reveal that it serves to replicate the strong interfacial magnetization found at the top and bottom interfaces. These results are of great value both in understanding the fundamental physics of such an order transition, and in considering FeRh(Pd) for magnetic media and spintronics applications. C1 [Bennett, S. P.; Lauter, V.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37830 USA. [Ambaye, H.] Oak Ridge Natl Lab, Res Accelerator Div, Oak Ridge, TN 37830 USA. [Lee, H.; LeClair, P.; Mankey, G. J.] Univ Alabama, Dept Phys & Astron, Tuscaloosa, AL 35487 USA. RP Bennett, SP (reprint author), Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37830 USA. EM bennettsp@ornl.gov RI Mankey, Gary/G-9110-2011; ambaye, haile/D-1503-2016 OI Mankey, Gary/0000-0003-3163-5159; ambaye, haile/0000-0002-8122-9952 FU DOE award [DE-FG02-08ER46499]; Scientific User Facilities Division, Office of Basic Energy Sciences, DOE FX S.B. thanks Dr. A. Glavic for helpful conversations on neutron reflectivity data fitting. H.L., P.L. and G.J.M. gratefully acknowledge financial support from DOE award DE-FG02-08ER46499. This work was supported by the Scientific User Facilities Division, Office of Basic Energy Sciences, DOE. NR 37 TC 4 Z9 4 U1 5 U2 50 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAR 16 PY 2015 VL 5 AR 9142 DI 10.1038/srep09142 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CD6DZ UT WOS:000351181000006 PM 25771919 ER PT J AU Shao, L Fu, EG Price, L Chen, D Chen, TY Wang, YQ Xie, GQ Lucca, DA AF Shao, Lin Fu, Engang Price, Lloyd Chen, Di Chen, Tianyi Wang, Yongqiang Xie, Guoqiang Lucca, Don A. TI Sink property of metallic glass free surfaces SO SCIENTIFIC REPORTS LA English DT Article ID INDUCED NANOCRYSTAL FORMATION; BULK AMORPHOUS-ALLOYS; MOLECULAR-DYNAMICS; FREE-VOLUME; IRRADIATION; TRANSFORMATION; TEMPERATURE; NUCLEATION; PRESSURE; DAMAGE AB When heated to a temperature close to glass transition temperature, metallic glasses (MGs) begin to crystallize. Under deformation or particle irradiation, crystallization occurs at even lower temperatures. Hence, phase instability represents an application limit for MGs. Here, we report that MG membranes of a few nanometers thickness exhibit properties different from their bulk MG counterparts. The study uses in situ transmission electron microscopy with concurrent heavy ion irradiation and annealing to observe crystallization behaviors of MGs. For relatively thick membranes, ion irradiations introduce excessive free volumes and thus induce nanocrystal formation at a temperature linearly decreasing with increasing ion fluences. For ultra-thin membranes, however, the critical temperature to initiate crystallization is about 100 K higher than the bulk glass transition temperature. Molecular dynamics simulations indicate that this effect is due to the sink property of the surfaces which can effectively remove excessive free volumes. These findings suggest that nanostructured MGs having a higher surface to volume ratio are expected to have higher crystallization resistance, which could pave new paths for materials applications in harsh environments requiring higher stabilities. C1 [Shao, Lin; Price, Lloyd; Chen, Di; Chen, Tianyi] Texas A&M Univ, Dept Nucl Engn, College Stn, TX 77843 USA. [Shao, Lin] Texas A&M Univ, Dept Mat Sci & Engn, College Stn, TX 77843 USA. [Fu, Engang] Peking Univ, Sch Phys, Beijing 100871, Peoples R China. [Wang, Yongqiang] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Xie, Guoqiang] Tohoku Univ, Inst Mat Res, Sendai, Miyagi 9808577, Japan. [Lucca, Don A.] Oklahoma State Univ, Sch Mech & Aerosp Engn, Stillwater, OK 74078 USA. RP Shao, L (reprint author), Texas A&M Univ, Dept Nucl Engn, College Stn, TX 77843 USA. EM lshao@tamu.edu; efu@pku.edu.cn RI Xie, Guoqiang/A-8619-2011; OI Chen, Tianyi/0000-0003-2880-824X FU National Science Foundation (USA) [1130589, 1130606] FX We acknowledge the financial support from the National Science Foundation (USA) through grants no.: 1130589 and no.: 1130606. NR 30 TC 1 Z9 1 U1 1 U2 52 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAR 16 PY 2015 VL 5 AR 8877 DI 10.1038/srep08877 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CD6DC UT WOS:000351178500001 PM 25777773 ER PT J AU Beck, AR Neumark, DM Leone, SR AF Beck, Annelise R. Neumark, Daniel M. Leone, Stephen R. TI Probing ultrafast dynamics with attosecond transient absorption SO CHEMICAL PHYSICS LETTERS LA English DT Article ID CHARGE MIGRATION; INDUCED TRANSPARENCY; SPECTROSCOPY; STATES; LIGHT; OSCILLATIONS; IONIZATION AB The broad bandwidth of an isolated attosecond pulse excites a vast number of states simultaneously, and the corresponding absorption features can be monitored with exceptional temporal resolution. Novel transient absorption experiments in gases using isolated attosecond pulses are performed in two regimes, one in which the attosecond pulse is overlapped in time with a near-infrared (NIR) pulse and one in which the NIR pulse follows the attosecond pulse. In the latter regime, the attosecond pulse first interacts with a sample, then the observed absorption features are modified by a NIR pulse, which interacts with the sample well after the attosecond pulse has passed. In these experiments, which seem counterintuitive when compared to conventional transient absorption spectroscopy, the weak attosecond pulse induces a polarization of the medium, which is then perturbed by the time-delayed NIR pulse. Recent measurements demonstrate the rich variety of information that can be extracted in this regime. (C) 2014 Elsevier B.V. All rights reserved. C1 [Beck, Annelise R.; Neumark, Daniel M.; Leone, Stephen R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Beck, Annelise R.; Neumark, Daniel M.; Leone, Stephen R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Ultrafast Xray Sci Lab, Berkeley, CA 94720 USA. [Leone, Stephen R.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. RP Beck, AR (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM annelise.r.beck@gmail.com RI Neumark, Daniel/B-9551-2009 OI Neumark, Daniel/0000-0002-3762-9473 FU Division of Chemical Sciences, Geosciences, and Biosciences of the U.S. Department of Energy at LBNL [DE-AC02-05CH11231]; National Science Foundation; Office of Assistant Secretary of Defense for Research and Engineering through a National Security Science and Engineering Faculty Fellowship FX This work was supported by the Director, Office of Science, Office of Basic Energy Sciences, and by the Division of Chemical Sciences, Geosciences, and Biosciences of the U.S. Department of Energy at LBNL under Contract No. DE-AC02-05CH11231. A.R.B. acknowledges funding from the National Science Foundation Graduate Research Fellowship Program. S.R.L. acknowledges the support of the Office of Assistant Secretary of Defense for Research and Engineering through a National Security Science and Engineering Faculty Fellowship. NR 41 TC 20 Z9 20 U1 5 U2 53 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2614 EI 1873-4448 J9 CHEM PHYS LETT JI Chem. Phys. Lett. PD MAR 16 PY 2015 VL 624 BP 119 EP 130 DI 10.1016/j.cplett.2014.12.048 PG 12 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CC5AK UT WOS:000350368500023 ER PT J AU Brunner, T Fudenberg, D Varentsov, V Sabourov, A Gratta, G Dilling, J DeVoe, R Sinclair, D Fairbank, W Albert, JB Auty, DJ Barbeau, PS Beck, D Benitez-Medina, C Breidenbach, M Cao, GF Chambers, C Cleveland, B Coon, M Craycraft, A Daniels, T Daugherty, SJ Didberidze, T Dolinski, MJ Dunford, M Fabris, L Farine, J Feldmeier, W Fierlinger, P Gornea, R Graham, K Heffner, M Hughes, M Jewell, M Jiang, XS Johnson, TN Johnston, S Karelin, A Kaufman, LJ Killick, R Koffas, T Kravitz, S Krucken, R Kuchenkov, A Kurnar, KS Leonard, DS Leonard, F Licciardi, C Lin, YH Ling, J MacLellan, R Marino, MG Mong, B Moore, D Odian, A Ostrovskiy, I Ouellet, C Piepke, A Pocar, A Retiere, F Rowson, PC Rozo, MP Schubert, A Smith, E Stekhanov, V Tarka, M Tolba, T Tosi, D Twelker, K Vuilleumier, JL Walton, J Walton, T Weber, M Wen, LJ Wichoski, U Yang, L Yen, YR AF Brunner, T. Fudenberg, D. Varentsov, V. Sabourov, A. Gratta, G. Dilling, J. DeVoe, R. Sinclair, D. Fairbank, W., Jr. Albert, J. B. Auty, D. J. Barbeau, P. S. Beck, D. Benitez-Medina, C. Breidenbach, M. Cao, G. F. Chambers, C. Cleveland, B. Coon, M. Craycraft, A. Daniels, T. Daugherty, S. J. Didberidze, T. Dolinski, M. J. Dunford, M. Fabris, L. Farine, J. Feldmeier, W. Fierlinger, P. Gornea, R. Graham, K. Heffner, M. Hughes, M. Jewell, M. Jiang, X. S. Johnson, T. N. Johnston, S. Karelin, A. Kaufman, L. J. Killick, R. Koffas, T. Kravitz, S. Kruecken, R. Kuchenkov, A. Kurnar, K. S. Leonard, D. S. Leonard, F. Licciardi, C. Lin, Y. H. Ling, J. MacLellan, R. Marino, M. G. Mong, B. Moore, D. Odian, A. Ostrovskiy, I. Ouellet, C. Piepke, A. Pocar, A. Retiere, F. Rowson, P. C. Rozo, M. P. Schubert, A. Smith, E. Stekhanov, V. Tarka, M. Tolba, T. Tosi, D. Twelker, K. Vuilleumier, J. -L. Walton, J. Walton, T. Weber, M. Wen, L. J. Wichoski, U. Yang, L. Yen, Y. -R. TI An RF-only ion-funnel for extraction from high-pressure gases SO INTERNATIONAL JOURNAL OF MASS SPECTROMETRY LA English DT Article DE RF-funnel; Gas dynamic and ion trajectory; simulations; Gas jet; Xe-136 double-beta decay; Ba tagging; Ion transport ID DOUBLE-BETA DECAY; MAJORANA NEUTRINOS; MASS-SPECTROMETER; SENSITIVITY; INTERFACE; TRAP; COMPUTER; EXO-200; XE AB An RF ion-funnel technique has been developed to extract ions from a high-pressure (10 bar) noble-gas environment into a vacuum (10(-6) mbar). Detailed simulations have been performed and a prototype has been developed for the purpose of extracting Ba-136 ions from Xe gas with high efficiency. With this prototype, ions have been extracted for the first time from high-pressure xenon gas and argon gas. Systematic studies have been carried out and compared to simulations. This demonstration of extraction of ions, with mass comparable to that of the gas generating the high-pressure, has applications to Ba tagging from a Xe-gas time-projection chamber for double-beta decay, as well as to the general problem of recovering trace amounts of an ionized element in a heavy (m > 40 u) carrier gas. (C) 2015 Elsevier B.V. All rights reserved. C1 [Brunner, T.; Fudenberg, D.; Sabourov, A.; Gratta, G.; DeVoe, R.; Jewell, M.; Kravitz, S.; Moore, D.; Ostrovskiy, I.; Schubert, A.; Tosi, D.; Twelker, K.; Weber, M.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Varentsov, V.; Karelin, A.; Kuchenkov, A.; Stekhanov, V.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Varentsov, V.] Facil Antiproton & Ion Res Europe FAIR GmbH, Darmstadt, Germany. [Dilling, J.; Sinclair, D.; Kruecken, R.; Retiere, F.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Sinclair, D.; Dunford, M.; Graham, K.; Killick, R.; Koffas, T.; Leonard, F.; Licciardi, C.; Ouellet, C.; Rozo, M. P.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. Colorado State Univ, Dept Phys, Ft Collins, CO 80523 USA. [Albert, J. B.; Daugherty, S. J.; Johnson, T. N.; Kaufman, L. J.] Indiana Univ, Dept Phys, Bloomington, IN USA. [Albert, J. B.; Daugherty, S. J.; Johnson, T. N.; Kaufman, L. J.] Indiana Univ, CEEM, Bloomington, IN USA. [Auty, D. J.; Didberidze, T.; Hughes, M.; Piepke, A.] Univ Alabama, Dept Phys & Astron, Tuscaloosa, AL 35487 USA. [Barbeau, P. S.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Barbeau, P. S.] TUNL, Durham, NC USA. [Beck, D.; Coon, M.; Ling, J.; Tarka, M.; Walton, J.; Yang, L.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Breidenbach, M.; Daniels, T.; Odian, A.; Rowson, P. C.] SIAC Natl Accelerator Lab, Menlo Pk, CA USA. [Cao, G. F.; Jiang, X. S.; Wen, L. J.] Inst High Energy Phys, Beijing 100039, Peoples R China. [Cleveland, B.; Mong, B.; Wichoski, U.] Laurentian Univ, Dept Phys, Sudbury, ON P3E 2C6, Canada. [Dolinski, M. J.; Smith, E.; Yen, Y. -R.] Drexel Univ, Dept Phys, Philadelphia, PA 19104 USA. [Fabris, L.] Oak Ridge Natl Lab, Oak Ridge, TN USA. [Feldmeier, W.; Fierlinger, P.; Marino, M. G.] Tech Univ Munich, Phys Dept & Excellence Cluster Universe, Garching, Germany. [Gornea, R.; Tolba, T.; Vuilleumier, J. -L.] Univ Bern, Albert Einstein Ctr, LHEP, Bern, Switzerland. [Heffner, M.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Johnston, S.; Pocar, A.] Univ Massachusetts, Amherst Ctr Fundamental Interact, Amherst, MA 01003 USA. [Johnston, S.; Pocar, A.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Kurnar, K. S.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Leonard, D. S.] Univ Seoul, Dept Phys, Seoul, South Korea. [MacLellan, R.] Univ S Dakota, Dept Phys, Vermillion, SD 57069 USA. RP Brunner, T (reprint author), Stanford Univ, Dept Phys, Stanford, CA 94305 USA. EM tbrunner@stanford.edu RI Fabris, Lorenzo/E-4653-2013; Kruecken, Reiner/A-1640-2013; OI Fabris, Lorenzo/0000-0001-5605-5615; Kruecken, Reiner/0000-0002-2755-8042; Ostrovskiy, Igor/0000-0003-4939-0225; Brunner, Thomas/0000-0002-3131-8148 FU US by NSF [PHY-0918469]; Russian Federation [RFBR 14-22-03028] FX This work was supported in the US by NSF grant PHY-0918469 and in the Russian Federation by grant RFBR 14-22-03028. NR 44 TC 2 Z9 2 U1 1 U2 22 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 1387-3806 EI 1873-2798 J9 INT J MASS SPECTROM JI Int. J. Mass Spectrom. PD MAR 15 PY 2015 VL 379 SI SI BP 110 EP 120 DI 10.1016/j.ijms.2015.01.003 PG 11 WC Physics, Atomic, Molecular & Chemical; Spectroscopy SC Physics; Spectroscopy GA CH0YK UT WOS:000353748100014 ER PT J AU van Stipdonk, MJ Patterson, K Gibson, JK Berden, G Oomens, J AF van Stipdonk, Michael J. Patterson, Khiry Gibson, John K. Berden, Giel Oomens, Jos TI IRMPD spectroscopy reveals a novel rearrangement reaction for modified peptides that involves elimination of the N-terminal amino acid SO INTERNATIONAL JOURNAL OF MASS SPECTROMETRY LA English DT Article DE IRMPD spectroscopy; Ion structure; Peptide fragmentation; Tandem MS; Collision-induced dissociation ID COLLISION-INDUCED DISSOCIATION; TANDEM MASS-SPECTROMETRY; MAIN FRAGMENTATION PATHWAYS; DENSITY-FUNCTIONAL THEORY; ALKALI-METAL ION; GAS-PHASE; PROTONATED PEPTIDES; INFRARED-SPECTROSCOPY; PRODUCT IONS; B(5) IONS AB In this study, peptides were derivatized by reaction with salicylaldehyde to create N-terminal imines (Schiff bases). Collision-induced dissociation of the imine-modified peptides produces a complete series of b and a ions (which reveal sequence). However, an unusual pathway is also observed, one that leads to elimination of the residue mass of the N-terminal amino acid despite the chemical modification to create the imine. This pathway was investigated further using infrared multiple-photon dissociation (IRMPD) spectroscopy and density functional theory with alanine-glycine-glycine (AGG) as the test peptide. The IRMPD spectrum for the product generated by loss of 71 from modified AGG (Sal-AGG) matches one predicted for protonated Sal-GG, as well as the IRMPD spectrum of glycine-glycine derivatized independently to produce a Schiff base. We conclude that the residue mass of the N-terminal amino acid is likely eliminated through a pathway that involves nucleophilic attack by an amide N atom and possible formation of an imidazole-4-one intermediate. (C) 2015 Elsevier B.V. All rights reserved. C1 [van Stipdonk, Michael J.; Patterson, Khiry] Duquesne Univ, Dept Chem & Biochem, Pittsburgh, PA 15282 USA. [Gibson, John K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Berden, Giel; Oomens, Jos] Radboud Univ Nijmegen, Inst Mol & Mat, FELIX Lab, NL-6525 ED Nijmegen, Netherlands. [Oomens, Jos] Univ Amsterdam, NL-1098 XH Amsterdam, Netherlands. RP van Stipdonk, MJ (reprint author), Duquesne Univ, Dept Chem & Biochem, 600 Forbes Ave, Pittsburgh, PA 15282 USA. EM vanstipdonkm@duq.edu RI Berden, Giel/F-9690-2015; Oomens, Jos/F-9691-2015 FU Duquesne University; Bayer School of Natural and Environmental Sciences; National Science Foundation [CHE-0963450]; U.S. Department of Energy, Office of Basic Energy Sciences, Heavy Element Chemistry, at LBNL [DE-AC02-05CH11231]; Netherlands Organisation for Scientific Research (NWO) [724.011.002]; Stichting Physica; National High Field FT-ICR Facility at the National High Magnetic Field Laboratory, Tallahassee, FL [CHE-9909502] FX MJV acknowledges support for this work in the form of startup funding from Duquesne University and the Bayer School of Natural and Environmental Sciences, and the National Science Foundation (CHE-0963450). The work of JKG was fully supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Heavy Element Chemistry, at LBNL under Contract No. DE-AC02-05CH11231. JO acknowledges the Netherlands Organisation for Scientific Research (NWO) for vici-grant no. 724.011.002 and the Stichting Physica. Construction and shipping of the FT-ICR-MS was made possible through funding from the National High Field FT-ICR Facility (grant CHE-9909502) at the National High Magnetic Field Laboratory, Tallahassee, FL. The excellent support by Dr. B. Redlich and others of the FELIX staff is gratefully acknowledged. NR 94 TC 4 Z9 4 U1 1 U2 20 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 1387-3806 EI 1873-2798 J9 INT J MASS SPECTROM JI Int. J. Mass Spectrom. PD MAR 15 PY 2015 VL 379 SI SI BP 165 EP 178 DI 10.1016/j.ijms.2015.01.010 PG 14 WC Physics, Atomic, Molecular & Chemical; Spectroscopy SC Physics; Spectroscopy GA CH0YK UT WOS:000353748100021 ER PT J AU Mamun, MA Gu, D Baumgart, H Elmustafa, AA AF Mamun, M. A. Gu, D. Baumgart, H. Elmustafa, A. A. TI Nanomechanical properties of platinum thin films synthesized by atomic layer deposition SO SURFACE & COATINGS TECHNOLOGY LA English DT Article DE Platinum thin films; ALD synthesis; TEM; XRD; AFM; Nanoindentation ID INSTRUMENTED INDENTATION AB The nanomechanical properties of Pt thin films grown on Si (100) using atomic layer deposition (ALD) were investigated using nanoindentation. Recently, atomic layer deposition (ALD) has successfully demonstrated the capability to deposit ultra-thin films of platinum (Pt). Using (methylcyclopentadienyl) trimethylplatinum (MeCpPtMe3) as chemical platinum precursor and oxygen (O-2) as the oxidizing agent, the ALD synthesis of Pt can be achieved with high conformity and excellent film uniformity. The ALD process window for Pt films was experimentally established in the temperature range between 270 degrees C and 320 degrees C, where the sheet conductance was constant over that temperature range, indicating stable ALD Pt film growth rate. ALD growth of Pt films exhibits very poor nucleation and adhesion characteristics on bare Si surfaces when the native oxide was removed by 2% HF etch. Pt adhesion improves for thermally oxidized Si wafers and for Si wafers covered with native oxide. Three ALD Pt films deposited at 800, 900, and 1000 ALD deposition cycles were tested for the structural and mechanical properties. Additionally, the sample with 900 ALD deposition cycles was further annealed in forming gas (95% N2 and 5% H-2) at 450 degrees C for 30 min in order to passivate dangling bonds in the grain boundaries of the polycrystalline Pt film. Cross-sectional transmission electron microscopy (TEM), X-ray diffraction (XRD), atomic force microscopy (AFM), and scanning electron microscope (SEM) were employed to characterize the films' surface structure and morphology. Nanoindentation technique was used to evaluate the hardness and modulus of the ALD Pt films of various film thicknesses. The results indicate that the films depict comparable hardness and modulus results; however, the 800 and 1000 ALD deposition cycles films without forming gas annealing experienced significant amount of pileup, whereas the 900 ALD deposition cycles sample annealed in forming gas resulted in a smaller pileup. (C) 2015 Elsevier B.V. All rights reserved. C1 [Mamun, M. A.; Elmustafa, A. A.] Old Dominion Univ, Dept Mech & Aerosp Engn, Norfolk, VA 23529 USA. [Gu, D.; Baumgart, H.] Old Dominion Univ, Dept Elect & Comp Engn, Norfolk, VA 23529 USA. [Mamun, M. A.; Gu, D.; Baumgart, H.; Elmustafa, A. A.] Thomas Jefferson Natl Accelerator Facil, Appl Res Ctr, Newport News, VA 23606 USA. RP Elmustafa, AA (reprint author), Old Dominion Univ, Dept Mech & Aerosp Engn, Norfolk, VA 23529 USA. EM aelmusta@odu.edu NR 17 TC 0 Z9 0 U1 4 U2 33 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0257-8972 J9 SURF COAT TECH JI Surf. Coat. Technol. PD MAR 15 PY 2015 VL 265 BP 185 EP 190 DI 10.1016/j.surfcoat.2015.01.037 PG 6 WC Materials Science, Coatings & Films; Physics, Applied SC Materials Science; Physics GA CF6MB UT WOS:000352669700023 ER PT J AU Yankeelov, TE Quaranta, V Evans, KJ Rericha, EC AF Yankeelov, Thomas E. Quaranta, Vito Evans, Katherine J. Rericha, Erin C. TI Toward a Science of Tumor Forecasting for Clinical Oncology SO CANCER RESEARCH LA English DT Article ID NEGATIVE BREAST-CANCER; NEOADJUVANT CHEMOTHERAPY; OVARIAN-CANCER; SURVIVAL; THERAPY; HETEROGENEITY; BEVACIZUMAB; MODEL AB We propose that the quantitative cancer biology community makes a concerted effort to apply lessons from weather forecasting to develop an analogous methodology for predicting and evaluating tumor growth and treatment response. Currently, the time course of tumor response is not predicted; instead, response is only assessed post hoc by physical examination or imaging methods. This fundamental practice within clinical oncology limits optimization of a treatment regimen for an individual patient, as well as to determine in real time whether the choice was in fact appropriate. This is especially frustrating at a time when a panoply of molecularly targeted therapies is available, and precision genetic or proteomic analyses of tumors are an established reality. By learning from the methods of weather and climate modeling, we submit that the forecasting power of biophysical and biomathematical modeling can be harnessed to hasten the arrival of a field of predictive oncology. With a successful methodology toward tumor forecasting, it should be possible to integrate large tumor-specific datasets of varied types and effectively defeat one cancer patient at a time. (C)2015 AACR. C1 [Yankeelov, Thomas E.] Vanderbilt Univ, Inst Imaging Sci, Nashville, TN 37232 USA. [Yankeelov, Thomas E.] Vanderbilt Univ, Dept Radiol & Radiol Sci, Nashville, TN 37232 USA. [Yankeelov, Thomas E.] Vanderbilt Univ, Dept Biomed Engn, Nashville, TN 37235 USA. [Yankeelov, Thomas E.; Rericha, Erin C.] Vanderbilt Univ, Dept Phys & Astron, Nashville, TN 37235 USA. [Yankeelov, Thomas E.; Quaranta, Vito] Vanderbilt Univ, Dept Canc Biol, Nashville, TN 37235 USA. [Yankeelov, Thomas E.; Quaranta, Vito] Vanderbilt Univ, Vanderbilt Ingram Canc Ctr, Nashville, TN 37235 USA. [Evans, Katherine J.] Oak Ridge Natl Lab, Comp Sci & Math Div, Nashville, TN USA. RP Yankeelov, TE (reprint author), Vanderbilt Univ, Inst Imaging Sci, Med Ctr, AA-1105 Med Ctr North,1161 21st Ave South, Nashville, TN 37232 USA. EM thomas.yankeelov@vanderbilt.edu RI Quaranta, Vito/G-6512-2016; OI Quaranta, Vito/0000-0001-7491-8672; Evans, Katherine/0000-0001-8174-6450 FU U.S. Department of Energy, Office of Science under the Scientific Discovery through Advanced Computing (SciDAC) project on Multiscale Methods for Accurate, Efficient, and Scale-Aware Models of the Earth System FX This work was supported in part by the U.S. Department of Energy, Office of Science under the Scientific Discovery through Advanced Computing (SciDAC) project on Multiscale Methods for Accurate, Efficient, and Scale-Aware Models of the Earth System. NR 36 TC 5 Z9 5 U1 1 U2 8 PU AMER ASSOC CANCER RESEARCH PI PHILADELPHIA PA 615 CHESTNUT ST, 17TH FLOOR, PHILADELPHIA, PA 19106-4404 USA SN 0008-5472 EI 1538-7445 J9 CANCER RES JI Cancer Res. PD MAR 15 PY 2015 VL 75 IS 6 BP 918 EP 923 DI 10.1158/0008-5472.CAN-14-2233 PG 6 WC Oncology SC Oncology GA CE6IZ UT WOS:000351941400003 PM 25592148 ER PT J AU Turner, WJN Walker, IS Roux, J AF Turner, W. J. N. Walker, I. S. Roux, J. TI Peak load reductions: Electric load shifting with mechanical pre-cooling of residential buildings with low thermal mass SO ENERGY LA English DT Article DE Pre-cooling; Load shifting; Air conditioning; Mechanical cooling; Peak demand; Thermal mass ID CONTROL STRATEGIES; ENERGY-SAVINGS; PERFORMANCE; WALLS; VENTILATION; CALIFORNIA; INSULATION; DESIGN; MODEL AB This study uses an advanced airflow, energy and humidity modelling tool to evaluate the potential for residential mechanical pre-cooling of building thermal mass to shift electricity loads away from the peak electricity demand period. The focus of this study is residential buildings with low thermal mass, such as timber-frame houses typical to the US. Simulations were performed for homes in 12 US DOE climate zones. The results show that the effectiveness of mechanical pre-cooling is highly dependent on climate zone and the selected pre-cooling strategy. The expected energy trade-off between cooling peak energy savings and increased off-peak energy use is also shown. The best pre-cooling results (more than 75% energy use shifted away from peak while minimising the total energy penalty) for most climates were obtained using a medium (5 h) pre-cooling time window with a shallow (23.3 degrees C) pre-cooling set point temperature. All of the pre-cooling strategies investigated caused the annual cooling energy demand of the simulated buildings to increase. Additionally, all of the pre-cooling strategies shifted at least 50% of the on-peak cooling loads away from a peak period window of 4pm-8pm in all climate zones. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Turner, W. J. N.; Walker, I. S.; Roux, J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Turner, W. J. N.] Univ Coll Dublin, Elect Res Ctr, Dublin 4, Ireland. [Roux, J.] Inst Natl Sci Appl, F-69621 Villeurbanne, France. RP Turner, WJN (reprint author), Univ Coll Dublin, Elect Res Ctr, Belfield Campus, Dublin 4, Ireland. EM will.turner@ucd.ie; iswalker@lbl.gov FU U.S. Dept. of Energy [DE-AC02-05CH11231] FX Funding for this work was provided by the U.S. Dept. of Energy under Contract No. DE-AC02-05CH11231. The authors would like to thank Karen Herter, Erin Hult and Vi Rapp for their help with this article. NR 58 TC 8 Z9 8 U1 2 U2 11 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-5442 EI 1873-6785 J9 ENERGY JI Energy PD MAR 15 PY 2015 VL 82 BP 1057 EP 1067 DI 10.1016/j.energy.2015.02.011 PG 11 WC Thermodynamics; Energy & Fuels SC Thermodynamics; Energy & Fuels GA CE4GI UT WOS:000351788700094 ER PT J AU Raugei, M Carbajales-Dale, M Barnhart, CJ Fthenakis, V AF Raugei, Marco Carbajales-Dale, Michael Barnhart, Charles J. Fthenakis, Vasilis TI Rebuttal: "Comments on 'Energy intensities, EROIs (energy returned on invested), and energy payback times of electricity generating power plants' - Making clear of quite some confusion" SO ENERGY LA English DT Editorial Material DE EROI (energy returned on invested); EROEI (energy returned on energy invested); Energy intensity; EPBT (Energy Pay-Back Time); Energy payback time; Life cycle assessment ID OIL C1 [Raugei, Marco] Oxford Brookes Univ, Fac Technol Design & Environm, Oxford OX33 1HX, England. [Raugei, Marco] Univ Pompeu Fabra, UNESCO, ESCI, Chair Life Cycle & Climate Change, Barcelona, Spain. [Raugei, Marco; Fthenakis, Vasilis] Columbia Univ, Ctr Life Cycle Anal, New York, NY USA. [Carbajales-Dale, Michael] Clemson Univ, Environm Engn & Earth Sci, Clemson, SC USA. [Barnhart, Charles J.] Western Washington Univ, Huxley Coll Environm, Dept Environm Sci, Bellingham, WA 98225 USA. [Fthenakis, Vasilis] Brookhaven Natl Lab, Photovolta Environm Res Ctr, Upton, NY 11973 USA. RP Raugei, M (reprint author), Oxford Brookes Univ, Fac Technol Design & Environm, Oxford OX33 1HX, England. EM marco.raugei@brookes.ac.uk RI Carbajales-Dale, Michael/I-7914-2015; Raugei, Marco/N-4737-2015 OI Carbajales-Dale, Michael/0000-0002-1568-384X; Raugei, Marco/0000-0001-5026-8556 NR 14 TC 4 Z9 4 U1 2 U2 8 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-5442 EI 1873-6785 J9 ENERGY JI Energy PD MAR 15 PY 2015 VL 82 BP 1088 EP 1091 DI 10.1016/j.energy.2014.12.060 PG 4 WC Thermodynamics; Energy & Fuels SC Thermodynamics; Energy & Fuels GA CE4GI UT WOS:000351788700096 ER PT J AU Inman, JL Robertson, C Mott, JD Bissell, MJ AF Inman, Jamie L. Robertson, Claire Mott, Joni D. Bissell, Mina J. TI Mammary gland development: cell fate specification, stem cells and the microenvironment SO DEVELOPMENT LA English DT Review DE MMPs; Mammary gland; Microenvironment; Progenitor cells; Stem cells ID LUMINAL PROGENITOR CELLS; BREAST EPITHELIAL-CELLS; EXTRACELLULAR-MATRIX; BRANCHING MORPHOGENESIS; BASEMENT-MEMBRANE; GENE-EXPRESSION; MYOEPITHELIAL CELLS; TRANSCRIPTION FACTOR; ADIPOCYTE DIFFERENTIATION; SELF-ORGANIZATION AB The development of the mammary gland is unique: the final stages of development occur postnatally at puberty under the influence of hormonal cues. Furthermore, during the life of the female, the mammary gland can undergo many rounds of expansion and proliferation. The mammary gland thus provides an excellent model for studying the 'stem/progenitor' cells that allow this repeated expansion and renewal. In this Review, we provide an overview of the different cell types that constitute the mammary gland, and discuss how these cell types arise and differentiate. As cellular differentiation cannot occur without proper signals, we also describe how the tissue microenvironment influences mammary gland development. C1 [Inman, Jamie L.; Robertson, Claire; Mott, Joni D.; Bissell, Mina J.] Univ Calif Berkeley, Div Life Sci, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Bissell, MJ (reprint author), Univ Calif Berkeley, Div Life Sci, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM mjbissell@lbl.gov FU Congressionally Directed Medical Research Programs of the US Department of Defense (DoD); Congressionally Directed Medical Research Programs of the DoD; Breast Cancer Research Foundation; National Cancer Institute; US Department of Energy Office of Biological and Environmental Research; Low Dose Radiation Program FX C.R. was supported by a fellowship from the Congressionally Directed Medical Research Programs of the US Department of Defense (DoD). M.J.B. was funded by Congressionally Directed Medical Research Programs of the DoD, The Breast Cancer Research Foundation and The National Cancer Institute. This work was also supported by the US Department of Energy Office of Biological and Environmental Research and Low Dose Radiation Program. NR 152 TC 34 Z9 35 U1 8 U2 36 PU COMPANY OF BIOLOGISTS LTD PI CAMBRIDGE PA BIDDER BUILDING CAMBRIDGE COMMERCIAL PARK COWLEY RD, CAMBRIDGE CB4 4DL, CAMBS, ENGLAND SN 0950-1991 EI 1477-9129 J9 DEVELOPMENT JI Development PD MAR 15 PY 2015 VL 142 IS 6 BP 1028 EP 1042 DI 10.1242/dev.087643 PG 15 WC Developmental Biology SC Developmental Biology GA CE3AY UT WOS:000351697700002 PM 25758218 ER PT J AU Choi, JH Chen, HL AF Choi, Jeong-Hoon Chen, Hung-Liang (Roger) TI Design of GFRP reinforced CRCP and its behavior sensitivity to material property variations SO CONSTRUCTION AND BUILDING MATERIALS LA English DT Article DE GFRP rebars; CRCP; Concrete shrinkage; Temperature variation; Bond-slip; Subbase; Crack spacing; Crack width ID SHRINKAGE; STRESSES AB Non-corrosiveness, light weight, and high strength-to-weight ratio of Glass Fiber Reinforced Polymer (GFRP) rebars would have favorable impacts on the Continuously Reinforced Concrete Pavements (CRCPs), in terms of lowering the maintenance cost and extending the longevity of the pavement. To examine the viability of GFRP rebars as CRCP's reinforcement, the U.S.'s first GFRP-CRCP test section Was constructed on Route 9 in Martinsburg, West Virginia, together with a conventional steel-CRCP test section for comparison purpose. In this paper, we introduce overall design methodology of these CRCP test sections, which involves mechanistic and numerical analyses. The reinforcement design of #7 longitudinal rebars at 6 in. (15.24 cm) spacing (1.0% ratio) is proposed to be mechanically and economically feasible for the GFRP-CRCP, when applied with 6500 psi (44.82 MPa) concrete on the cement-stabilized subbase. For the GFRP-CRCP design, shrinkage and thermal properties of concrete appear to be the most influential design parameters to the performance of the proposed GFRP-CRCP. Even though the actual field performance of the CRCP test sections shows appreciable discrepancy with its prediction, it still remains within the allowable limit for structural integrity. The properties of subbase and concrete deviating from their proposed design is presumably the cause of the discrepancy. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Choi, Jeong-Hoon] US DOE, AECOM, Natl Energy Technol Lab, Morgantown, WV 26507 USA. [Chen, Hung-Liang (Roger)] W Virginia Univ, Dept Civil & Environm Engn, Morgantown, WV 26506 USA. RP Choi, JH (reprint author), US DOE, AECOM, Natl Energy Technol Lab, Morgantown, WV 26507 USA. EM Jeong.Choi@contr.netl.doe.gov; Roger.Chen@mail.wvu.edu OI Chen, Hung-Liang/0000-0002-4278-5593 FU USDOT/FHWA [DTFH61-99-X-00078] FX This article is written based on the study supported by USDOT/FHWA (DTFH61-99-X-00078). The authors gratefully acknowledge Peter Kopac and Sam Tyson of FHWA for their valuable comments and support. Appreciation is also extended to Dr. Hota V. GangaRao and Dr. P.V. Vijay of the Constructed Facility Center at West Virginia University for their assistance during this study. NR 32 TC 0 Z9 0 U1 1 U2 8 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0950-0618 EI 1879-0526 J9 CONSTR BUILD MATER JI Constr. Build. Mater. PD MAR 15 PY 2015 VL 79 BP 420 EP 432 DI 10.1016/j.conbuildmat.2014.12.080 PG 13 WC Construction & Building Technology; Engineering, Civil; Materials Science, Multidisciplinary SC Construction & Building Technology; Engineering; Materials Science GA CD2RR UT WOS:000350927200047 ER PT J AU Huie, MM Bock, DC Takeuchi, ES Marschilok, AC Takeuchi, KJ AF Huie, Matthew M. Bock, David C. Takeuchi, Esther S. Marschilok, Amy C. Takeuchi, Kenneth J. TI Cathode materials for magnesium and magnesium-ion based batteries SO COORDINATION CHEMISTRY REVIEWS LA English DT Review DE Magnesium battery; Magnesium-ion battery; Energy storage; Cathode material ID RECHARGEABLE MG BATTERIES; VANADIUM-OXIDE NANOTUBES; MO6S8 CHEVREL-PHASE; ELECTROCHEMICAL INSERTION; CRYSTAL-STRUCTURE; POLYVALENT CATIONS; MGXMO6T8 T; STRUCTURAL-CHARACTERIZATION; INTERCALATION PROPERTIES; APROTIC ELECTROLYTES AB Rechargeable magnesium-ion batteries are a promising candidate technology to address future electrical energy storage needs of large scale mobile and stationary devices, due to the high environmental abundance of magnesium metal and divalent character of magnesium ion. With the recent increase in reports discussing cathode materials for magnesium-ion batteries, it is instructive to assess recent research in order to provide inspiration for future research. This review is a summary of the different chemistries and structures of the materials developed for magnesium ion cathodes. The particular strategies which may lead to future research initiatives are amplified. (C) 2014 Elsevier B.V. All rights reserved. C1 [Huie, Matthew M.; Takeuchi, Esther S.; Marschilok, Amy C.; Takeuchi, Kenneth J.] SUNY Stony Brook, Dept Mat Sci & Engn, Stony Brook, NY 11794 USA. [Bock, David C.; Takeuchi, Esther S.; Marschilok, Amy C.; Takeuchi, Kenneth J.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Takeuchi, Esther S.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Takeuchi, KJ (reprint author), SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. EM kenneth.takeuchi.1@stonybrook.edu FU Department of Energy, Office of Electricity [1275961] FX The authors gratefully acknowledge support by the Department of Energy, Office of Electricity, administered through Sandia National Laboratories, Purchase Order #1275961. NR 113 TC 37 Z9 37 U1 74 U2 404 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0010-8545 EI 1873-3840 J9 COORDIN CHEM REV JI Coord. Chem. Rev. PD MAR 15 PY 2015 VL 287 BP 15 EP 27 DI 10.1016/j.ccr.2014.11.005 PG 13 WC Chemistry, Inorganic & Nuclear SC Chemistry GA CD2RC UT WOS:000350925700002 ER PT J AU Portenga, EW Bierman, PR Duncan, C Corbett, LB Kehrwald, NM Rood, DH AF Portenga, Eric W. Bierman, Paul R. Duncan, Chris Corbett, Lee B. Kehrwald, Natalie M. Rood, Dylan H. TI Erosion rates of the Bhutanese Himalaya determined using in situ-produced Be-10 SO GEOMORPHOLOGY LA English DT Article DE Bhutan; Sediment; Cosmogenic nuclide; Denudation; Uplift; Beryllium ID LONG-TERM EROSION; COSMOGENIC NUCLIDES; DENUDATION RATES; THRESHOLD HILLSLOPES; LANDSCAPE EVOLUTION; FIELD-MEASUREMENTS; BOLIVIAN ANDES; NORTHERN CHILE; AMS STANDARDS; FROST ACTION AB Western Bhutan provides an ideal setting to understand the interplay between uplift, erosion, and fluvial sediment transport in an active mountain environment. Using in situ-produced Be-10 (49 samples) and Al-26 (5 samples) in fluvial sediment from nested catchments throughout the Puna Tsang Chhu drainage basin, we examine erosion rates in different geomorphic environments including two high-relief regions - a glacierized zone in the north and a high-rainfall zone in the south - as well as remnants of an uplifted, lower-relief paleosurface between them. The erosion rates roughly mirror this north-south zonation: lower rates (avg. 388 +/- 32 m My(-1), n = 16) prevail in the low-relief zone, roughly coinciding with lower-relief terrain where mean annual precipitation is similar to 1500 mm yr(-1); the highest rates (avg. 956 +/- 160 m My(-1), n = 13) are in the south (27.10 degrees-2735 degrees N), where rainfall is >4000 mm yr(-1); high rates (avg. 700 +/- 62 m My(-1), n = 15) also occur in the northern, glacierized region (27.70 degrees-28.10 degrees N). All 49 purified mineral separates used in this study contain measurable amounts of native Be-9 (up to 900 mu g), violating the assumption of negligible 9Be that is commonly made in the isotope dilution method used to quantify Be-10. To correct for this native 9Be, we use high precision, replicate measurements of Be-9 in each sample to calculate Be-10 concentrations from measured isotopic ratios. Neglecting native Be-9 would have led to erosion rate overestimates from <20% to >400%. The pervasive nature of 9Be in these samples underscores the importance of quantifying the native 9Be concentration in mineral separates used for cosmogenic Be-9 analysis. (C) 2014 Elsevier B.V. All rights reserved. C1 [Portenga, Eric W.] Univ Glasgow, Sch Geog & Earth Sci, Glasgow G12 8QQ, Lanark, Scotland. [Portenga, Eric W.] Macquarie Univ, Dept Geog & Environm, Sydney, NSW 2109, Australia. [Bierman, Paul R.; Corbett, Lee B.] Univ Vermont, Dept Geol, Burlington, VT 05405 USA. [Bierman, Paul R.; Corbett, Lee B.] Univ Vermont, Rubenstein Sch Environm & Nat Resources, Burlington, VT 05405 USA. [Duncan, Chris] Univ Massachusetts, Dept Geosci, Amherst, MA 01002 USA. [Kehrwald, Natalie M.] Ca Foscari Univ Venice, Dept Environm Sci Informat & Stat, I-30123 Venice, Italy. [Rood, Dylan H.] Univ London Imperial Coll Sci Technol & Med, Dept Earth Sci & Engn, London SW7 2AZ, England. [Rood, Dylan H.] Lawrence Livermore Natl Lab, Ctr Accelerator Mass Spectrometry, Livermore, CA 94550 USA. RP Portenga, EW (reprint author), Univ Glasgow, Sch Geog & Earth Sci, Glasgow G12 8QQ, Lanark, Scotland. EM e.portenga.1@research.gla.ac.uk; pbierman@uvm.edu; duncan@gismatters.com; abcorbet@uvm.edu; kehrwald@unive.it; d.rood@imperial.ac.uk RI Kehrwald, Natalie/A-3848-2013 OI Kehrwald, Natalie/0000-0002-9160-2239 FU National Aeronautical and Space Administration [NAGS 10649] FX We thank J. Masek for productive discussions and suggestions, D. Grujic for collecting samples in 2000, and two anonymous reviewers for constructive reviews, insights, advice, and suggestions. Sample collection (2002 only) and processing (all years) were supported by National Aeronautical and Space Administration grant NAGS 10649. NR 108 TC 8 Z9 8 U1 1 U2 21 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0169-555X EI 1872-695X J9 GEOMORPHOLOGY JI Geomorphology PD MAR 15 PY 2015 VL 233 SI SI BP 112 EP 126 DI 10.1016/j.geomorph.2014.09.027 PG 15 WC Geography, Physical; Geosciences, Multidisciplinary SC Physical Geography; Geology GA CC6ZM UT WOS:000350517500009 ER PT J AU Singha, K Day-Lewis, FD Johnson, T Slater, LD AF Singha, K. Day-Lewis, F. D. Johnson, T. Slater, L. D. TI Advances in interpretation of subsurface processes with time-lapse electrical imaging SO HYDROLOGICAL PROCESSES LA English DT Review DE electrical resistivity; induced polarization; complex resistivity; imaging; petrophysics; inversion ID INDUCED-POLARIZATION DATA; DATA INCORPORATING TOPOGRAPHY; NONSYMMETRIC LINEAR-SYSTEMS; INFILTRATING RIVER WATER; RESISTIVITY TOMOGRAPHY; SOLUTE TRANSPORT; RESISTANCE TOMOGRAPHY; DC-RESISTIVITY; COMPLEX CONDUCTIVITY; VADOSE ZONE AB Electrical geophysical methods, including electrical resistivity, time-domain induced polarization, and complex resistivity, have become commonly used to image the near subsurface. Here, we outline their utility for time-lapse imaging of hydrological, geochemical, and biogeochemical processes, focusing on new instrumentation, processing, and analysis techniques specific to monitoring. We review data collection procedures, parameters measured, and petrophysical relationships and then outline the state of the science with respect to inversion methodologies, including coupled inversion. We conclude by highlighting recent research focused on innovative applications of time-lapse imaging in hydrology, biology, ecology, and geochemistry, among other areas of interest. Copyright (c) 2014 John Wiley & Sons, Ltd. C1 [Singha, K.] Colorado Sch Mines, Hydrol Sci & Engn Program, Golden, CO 80401 USA. [Day-Lewis, F. D.] US Geol Survey, Off Groundwater, Branch Geophys, Storrs, CT 06269 USA. [Johnson, T.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Slater, L. D.] Rutgers State Univ, Dept Earth & Environm Sci, Newark, NJ 07102 USA. RP Singha, K (reprint author), Colorado Sch Mines, Hydrol Sci & Engn Program, Golden, CO 80401 USA. EM ksingha@mines.edu OI Day-Lewis, Frederick/0000-0003-3526-886X FU National Science Foundation [EAR-0747629]; Environmental Protection Agency Region 1; U.S. Geological Survey's Toxic Substances Hydrology Program; U.S. Geological Survey's Groundwater Resources Program FX This research was supported in part by National Science Foundation Grant EAR-0747629 and Environmental Protection Agency Region 1 and the U.S. Geological Survey's Toxic Substances Hydrology Program and Groundwater Resources Program. We thank two anonymous reviews and Burke Minsley for thoughtful feedback. Any use of trade, firm, or product names is for descriptive purposes only and does not imply endorsement by the US Government. NR 212 TC 18 Z9 19 U1 7 U2 37 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0885-6087 EI 1099-1085 J9 HYDROL PROCESS JI Hydrol. Process. PD MAR 15 PY 2015 VL 29 IS 6 BP 1549 EP 1576 DI 10.1002/hyp.10280 PG 28 WC Water Resources SC Water Resources GA CC7LD UT WOS:000350548100056 ER PT J AU Kim, D Ward, DR Simmons, CB Gamble, JK Blume-Kohout, R Nielsen, E Savage, DE Lagally, MG Friesen, M Coppersmith, SN Eriksson, MA AF Kim, Dohun Ward, D. R. Simmons, C. B. Gamble, John King Blume-Kohout, Robin Nielsen, Erik Savage, D. E. Lagally, M. G. Friesen, Mark Coppersmith, S. N. Eriksson, M. A. TI Microwave-driven coherent operation of a semiconductor quantum dot charge qubit SO NATURE NANOTECHNOLOGY LA English DT Article ID SINGLE-ELECTRON SPIN; COMPUTATION; CIRCUIT AB An intuitive realization of a qubit is an electron charge at two well-defined positions of a double quantum dot. This qubit is simple and has the potential for high-speed operation because of its strong coupling to electric fields. However, charge noise also couples strongly to this qubit, resulting in rapid dephasing at all but one special operating point called the ` sweet spot'. In previous studies d.c. voltage pulses have been used to manipulate semiconductor charge qubits(1-8) but did not achieve high-fidelity control, because d.c. gating requires excursions away from the sweet spot. Here, by using resonant a. c. microwave driving we achieve fast (greater than gigahertz) and universal single qubit rotations of a semiconductor charge qubit. The Z-axis rotations of the qubit are well protected at the sweet spot, and we demonstrate the same protection for rotations about arbitrary axes in the X-Y plane of the qubit Bloch sphere. We characterize the qubit operation using two tomographic approaches: standard process tomography(9,10) and gate set tomography(11). Both methods consistently yield process fidelities greater than 86% with respect to a universal set of unitary single-qubit operations. C1 [Kim, Dohun; Ward, D. R.; Simmons, C. B.; Friesen, Mark; Coppersmith, S. N.; Eriksson, M. A.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Gamble, John King; Blume-Kohout, Robin; Nielsen, Erik] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Savage, D. E.; Lagally, M. G.] Univ Wisconsin, Dept Mat Sci & Engn, Madison, WI 53706 USA. RP Eriksson, MA (reprint author), Univ Wisconsin, Dept Phys, 1150 Univ Ave, Madison, WI 53706 USA. EM maeriksson@wisc.edu OI Friesen, Mark/0000-0003-2878-2844 FU Army Research Office [W911NF-12-0607]; National Science Foundation [PHY-1104660]; Laboratory Directed Research and Development programme at Sandia National Laboratories; United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; Department of Energy [DE-FG02-03ER46028]; National Science Foundation FX This work was supported in part by the Army Research Office (W911NF-12-0607), the National Science Foundation (PHY-1104660) and by the Laboratory Directed Research and Development programme at Sandia National Laboratories. Sandia National Laboratories is a multi-programme laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the United States Department of Energy's National Nuclear Security Administration (contract DE-AC04-94AL85000). Development and maintenance of the growth facilities used for fabricating samples is supported by the Department of Energy (DE-FG02-03ER46028). This research utilized National Science Foundation-supported shared facilities at the University of Wisconsin-Madison. NR 30 TC 14 Z9 14 U1 1 U2 42 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1748-3387 EI 1748-3395 J9 NAT NANOTECHNOL JI Nat. Nanotechnol. PD MAR 15 PY 2015 VL 10 IS 3 BP 243 EP 247 DI 10.1038/NNANO.2014.336 PG 5 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA CD0YG UT WOS:000350799700015 PM 25686478 ER PT J AU Ruiz-Riol, M Llano, A Ibarrondo, J Zamarreno, J Yusim, K Bach, V Mothe, B Perez-Alvarez, S Fernandez, MA Requena, G Meulbroek, M Pujol, F Leon, A Cobarsi, P Korber, BT Clotet, B Ganoza, C Sanchez, J Coll, J Brander, C AF Ruiz-Riol, Marta Llano, Anuska Ibarrondo, Javier Zamarreno, Jennifer Yusim, Karina Bach, Vanessa Mothe, Beatriz Perez-Alvarez, Susana Fernandez, Marco A. Requena, Gerard Meulbroek, Michael Pujol, Ferran Leon, Agathe Cobarsi, Patricia Korber, Bette T. Clotet, Bonaventura Ganoza, Carmela Sanchez, Jorge Coll, Josep Brander, Christian TI Alternative Effector-Function Profiling Identifies Broad HIV-Specific T-Cell Responses in Highly HIV-Exposed Individuals Who Remain Uninfected SO JOURNAL OF INFECTIOUS DISEASES LA English DT Article DE boosted flow cytometry; highly exposed seronegative; HIV infection; toggled peptides; T-cell responses; Th1 cytokines; Th2 cytokines; Th17 cytokines ID HUMAN-IMMUNODEFICIENCY-VIRUS; HOST-RESISTANCE; VIRAL DIVERSITY; INFECTION; ACTIVATION; IMMUNE; SUSCEPTIBILITY; DESIGN; LEVEL; CD4 AB The characterization of host immune responses to human immunodeficiency virus (HIV) in HIV controllers and individuals with high exposure but seronegativity to HIV (HESN) is needed to guide the development of effective preventive and therapeutic vaccine candidates. However, several technical hurdles severely limit the definition of an effective virus-specific T-cell response. By using a toggle-peptide approach, which takes HIV sequence diversity into account, and a novel, boosted cytokine staining/flow cytometry strategy, we here describe new patterns of T-cell responses to HIV that would be missed by standard assays. Importantly, this approach also allows detection of broad and strong virus-specific T-cell responses in HESN individuals that are characterized by a T-helper type 1 cytokine-like effector profile and produce cytokines that have been associated with potential control of HIV infection, including interleukin 10, interleukin 13, and interleukin 22. These results establish a novel approach to improve the current understanding of HIV-specific T-cell immunity and identify cellular immune responses and individual cytokines as potential markers of relative HIV resistance. As such, the findings also help develop similar strategies for more-comprehensive assessments of host immune responses to other human infections and immune-mediated disorders. C1 [Ruiz-Riol, Marta; Llano, Anuska; Zamarreno, Jennifer; Bach, Vanessa; Mothe, Beatriz; Clotet, Bonaventura; Coll, Josep; Brander, Christian] Autonomous Univ Barcelona, Irsicaixa AIDS Res Inst, HIVACAT, Badalona, Spain. [Mothe, Beatriz; Cobarsi, Patricia; Clotet, Bonaventura; Coll, Josep] Hosp Badalona Germans Trias & Pujol, Fundacio Lluita Contra La Sida, Badalona, Spain. [Fernandez, Marco A.; Requena, Gerard] Hlth Sci Res Inst Germans Trias & Pujol, Flow Cytometry Facil, Badalona, Spain. [Perez-Alvarez, Susana] Biokit Res & Dev, Llica Damunt, Spain. [Meulbroek, Michael; Pujol, Ferran] Projecte NOMS Hispanosida, BCN Checkpoint, Barcelona, Spain. [Leon, Agathe] Hosp Clin Barcelona, Fundacio Clin, HIVACAT, Barcelona, Spain. [Brander, Christian] Inst Catalana Recerca & Estudis Avancats ICREA, Barcelona, Spain. [Mothe, Beatriz; Clotet, Bonaventura; Brander, Christian] Univ Vic, Barcelona, Spain. [Ibarrondo, Javier] Univ Calif Los Angeles, Ctr HIV Prevent Res, Los Angeles, CA 90024 USA. [Yusim, Karina; Korber, Bette T.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Ganoza, Carmela; Sanchez, Jorge] Asociac Civil Impacta Salud & Educ, Lima, Peru. RP Brander, C (reprint author), Hosp Badalona Germans Trias & Pujol, Lab Retrovirol, Fundacio IrsiCaixa, Ctra Canyet S-N, Barcelona 08916, Catalonia, Spain. EM cbrander@irsicaixa.es OI Brander, Christian/0000-0002-0548-5778; Korber, Bette/0000-0002-2026-5757; Fernandez, Marco A/0000-0002-3921-2209 FU HIVACAT program; FIS [PS0900283, FIPSE36-0737-09]; European Community (CUT'HIVAC) [EC-7FP-241904]; National Institutes of Health [R01 DE018925-05]; ISCIII (Rio Hortega) [CM08/00020, JR13/00024]; Institucio Catalana de Recerca I Estudis Avancats; Barcelona HIV Gala FX This work was supported by the HIVACAT program, the FIS (grants PS0900283 and FIPSE36-0737-09 to C. B.), the European Community (CUT'HIVAC; grant EC-7FP-241904 to C. B.), the National Institutes of Health (grant R01 DE018925-05 to C. B.), the ISCIII (Rio Hortega; grants CM08/00020 and JR13/00024 to B. M.), the Institucio Catalana de Recerca I Estudis Avancats (to C. B.), an unrestricted donation by Rafael Punter, and the Barcelona HIV Gala 2012. NR 36 TC 3 Z9 3 U1 2 U2 4 PU OXFORD UNIV PRESS INC PI CARY PA JOURNALS DEPT, 2001 EVANS RD, CARY, NC 27513 USA SN 0022-1899 EI 1537-6613 J9 J INFECT DIS JI J. Infect. Dis. PD MAR 15 PY 2015 VL 211 IS 6 BP 936 EP 946 DI 10.1093/infdis/jiu534 PG 11 WC Immunology; Infectious Diseases; Microbiology SC Immunology; Infectious Diseases; Microbiology GA CC3CX UT WOS:000350223300012 PM 25249264 ER PT J AU Harrup, MK Rollins, HW Jamison, DK Dufek, EJ Gering, KL Luther, TA AF Harrup, Mason K. Rollins, Harry W. Jamison, David K. Dufek, Eric J. Gering, Kevin L. Luther, Thomas A. TI Unsaturated phosphazenes as co-solvents for lithium-ion battery electrolytes SO JOURNAL OF POWER SOURCES LA English DT Article DE Phosphazene; Electrolytes; Lithium-ion battery; Unsaturated ID SAFE; PERFORMANCE; ADDITIVES; CARBONATE; LIQUID; CELLS AB This paper covers the synthesis and use of a related family of cyclic phosphazene solvents containing terminal unsaturations that are being considered as electrolyte additives in lithium-ion cells. A brief synopsis on the synthesis and purification of these compounds is given. Data will be presented that covers physical and chemical properties of the phosphazenes as well as the properties when blended at various levels with representative organic carbonate baseline solvents. Electrochemical cycling data will be presented using commercially available electrode couples as well as studies focusing on cell performance at early lifetime as well as after repeated cycles. Conclusions regarding the effect of the unsaturated phosphazene compounds and their interaction with various alkyl carbonates, and their effect on cell performance will be presented. (C) 2014 Elsevier B.V. All rights reserved. C1 [Harrup, Mason K.; Rollins, Harry W.; Jamison, David K.; Dufek, Eric J.; Gering, Kevin L.; Luther, Thomas A.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. RP Rollins, HW (reprint author), Idaho Natl Lab, POB 1625, Idaho Falls, ID 83415 USA. EM harry.rollins@inl.gov RI Rollins, Harry/B-6327-2017; Dufek, Eric/B-8847-2017 OI Rollins, Harry/0000-0002-3926-7445; Dufek, Eric/0000-0003-4802-1997 FU Idaho National Laboratory [DE-AC07-051D14517] FX The authors gratefully acknowledge Peter Faguy and David Howell and the Office of Energy Efficiency and Renewable Energy, ABR Program within the United States Department of Energy. The authors also acknowledge support from the Idaho National Laboratory per contract DE-AC07-051D14517. NR 20 TC 4 Z9 5 U1 2 U2 41 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD MAR 15 PY 2015 VL 278 BP 794 EP 801 DI 10.1016/j.jpowsour.2014.07.109 PG 8 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA CC2NH UT WOS:000350181400095 ER PT J AU Zhang, LL Duan, S Yang, XL Liang, G Huang, YH Cao, XZ Yang, J Li, M Croft, MC Lewis, C AF Zhang, Lu-Lu Duan, Song Yang, Xue-Lin Liang, Gan Huang, Yun-Hui Cao, Xing-Zhong Yang, Jing Li, Ming Croft, Mark C. Lewis, Cale TI Insight into cobalt-doping in Li2FeSiO4 cathode material for lithium-ion battery (vol 274C, pg 194, 2014) SO JOURNAL OF POWER SOURCES LA English DT Correction C1 [Zhang, Lu-Lu; Duan, Song; Yang, Xue-Lin; Li, Ming] China Three Gorges Univ, Coll Mat & Chem Engn, Hubei Prov Collaborat Innovat Ctr New Energy Micr, Yichang 443002, Hubei, Peoples R China. [Zhang, Lu-Lu] Chinese Acad Sci, Shanghai Inst Ceram, CAS Key Lab Mat Energy Convers, Shanghai 200050, Peoples R China. [Liang, Gan; Lewis, Cale] Sam Houston State Univ, Dept Phys, Huntsville, TX 77341 USA. [Huang, Yun-Hui] Huazhong Univ Sci & Technol, Sch Mat Sci & Engn, State Key Lab Mat Proc & Die & Mould Technol, Wuhan 430074, Hubei, Peoples R China. [Cao, Xing-Zhong; Yang, Jing] Chinese Acad Sci, Key Lab Nucl Anal Tech, Inst High Energy Phys, Beijing 100049, Peoples R China. [Croft, Mark C.] Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08854 USA. [Croft, Mark C.] Brookhaven Natl Lab, NSLS, Upton, NY 11973 USA. RP Yang, XL (reprint author), China Three Gorges Univ, Coll Mat & Chem Engn, Hubei Prov Collaborat Innovat Ctr New Energy Micr, 8 Daxue Rd, Yichang 443002, Hubei, Peoples R China. EM xlyang@ctgu.edu.cn NR 1 TC 0 Z9 0 U1 3 U2 37 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD MAR 15 PY 2015 VL 278 BP 826 EP 827 DI 10.1016/j.jpowsour.2014.12.115 PG 2 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA CC2NH UT WOS:000350181400098 ER PT J AU Bevc, S Junghans, C Praprotnik, M AF Bevc, Stas Junghans, Christoph Praprotnik, Matej TI STOCK: Structure Mapper and Online Coarse-Graining Kit for Molecular Simulations SO JOURNAL OF COMPUTATIONAL CHEMISTRY LA English DT Article DE coarse-graining; molecular simulations; iterative Boltzmann; structure mapping; web tool ID MULTISCALE SIMULATIONS; ADAPTIVE RESOLUTION; SOFTWARE PACKAGE; FORCE-FIELD; DYNAMICS; POTENTIALS; SYSTEMS; MODEL; WATER; PROGRAM AB We present a web toolkit STructure mapper and Online Coarse-graining Kit for setting up coarse-grained molecular simulations. The kit consists of two tools: structure mapping and Boltzmann inversion tools. The aim of the first tool is to define a molecular mapping from high, for example, all-atom, to low, that is, coarse-grained, resolution. Using a graphical user interface it generates input files, which are compatible with standard coarse-graining packages, for example, Versatile Object-oriented Toolkit for Coarse-graining Applications and DL_CGMAP. Our second tool generates effective potentials for coarse-grained simulations preserving the structural properties, for example, radial distribution functions, of the underlying higher resolution model. The required distribution functions can be provided by any simulation package. Simulations are performed on a local machine and only the distributions are uploaded to the server. The applicability of the toolkit is validated by mapping atomistic pentane and polyalanine molecules to a coarse-grained representation. Effective potentials are derived for systems of TIP3P (transferable intermolecular potential 3 point) water molecules and salt solution. The presented coarse-graining web toolkit is available at . (c) 2014 Wiley Periodicals, Inc. C1 [Bevc, Stas; Praprotnik, Matej] Natl Inst Chem, Lab Mol Modeling, SI-1001 Ljubljana, Slovenia. [Junghans, Christoph] Los Alamos Natl Lab, Comp Computat & Stat Sci Div, Los Alamos, NM 87545 USA. RP Bevc, S (reprint author), Natl Inst Chem, Lab Mol Modeling, Hajdrihova 19, SI-1001 Ljubljana, Slovenia. EM stas.bevc@cmm.ki.si RI Junghans, Christoph/G-4238-2010 OI Junghans, Christoph/0000-0003-0925-1458 FU Slovenian Research Agency [J1-4134, P1-0002]; U.S. DOE [DE-AC52-06NA25396] FX Contract grant sponsor: Slovenian Research Agency (S.B., M.P.); Contract grant number: J1-4134 and P1-0002; Contract grant sponsor: LANL is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. DOE; Contract grant number: DE-AC52-06NA25396 NR 54 TC 4 Z9 4 U1 2 U2 16 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0192-8651 EI 1096-987X J9 J COMPUT CHEM JI J. Comput. Chem. PD MAR 15 PY 2015 VL 36 IS 7 BP 467 EP 477 DI 10.1002/jcc.23806 PG 11 WC Chemistry, Multidisciplinary SC Chemistry GA CC0ZA UT WOS:000350067400007 PM 25504076 ER PT J AU Chen, JJ Mason, JA Bloch, ED Gygi, D Long, JR Reimer, JA AF Chen, Joseph J. Mason, Jarad A. Bloch, Eric D. Gygi, David Long, Jeffrey R. Reimer, Jeffrey A. TI NMR relaxation and exchange in metal-organic frameworks for surface area screening SO MICROPOROUS AND MESOPOROUS MATERIALS LA English DT Article; Proceedings Paper CT 12th International Bologna Conference on Magnetic Resonance in Porous Media (MRPM) CY FEB 09-13, 2014 CL Victoria Univ Wellington, Fac Sci, Wellington, NEW ZEALAND SP Magritek Ltd, Bruker BioSpin GmbH, MR Solut Ltd, Oxford Instruments, Schlumberger Doll Res, Stelar srl, HTS 110, Pure Devices, Shell, Tecmag, MacDiarmid Inst, Univ Bologna, Univ Wellington HO Victoria Univ Wellington, Fac Sci DE Metal-organic frameworks; NMR relaxometry; Exchange; High-throughput screening ID ZEOLITIC IMIDAZOLATE FRAMEWORKS; HIGH-THROUGHPUT SYNTHESIS; CARBON-DIOXIDE; COORDINATION POLYMER; HYDROGEN STORAGE; CAPTURE; ADSORPTION; PORES; MOF-5 AB We describe a robust screening technique that correlates the surface area of metal organic frameworks to the proton T-2 relaxation behavior of imbibed solvent at low field (13 MHz). In frameworks with small pore sizes (<1 nm) or strong solvent-framework interactions, diffusional exchange between the pore-confined and inter-particle solvent populations remains slow compared to the T-2 of the pore-confined solvent, allowing for a direct porosity analysis of the T-2 spectrum obtained from Laplace inversions. Increases in framework pore-size (>1 nm) lead to corresponding increases in the rate of solvent exchange, as confirmed by T-2 relaxation exchange (REXSY) experiments; increases in the pore size also increases the T-2 of the pore-confined solvent. The combination of these two effects results in comparable rates of relaxation and exchange, which precludes the direct analysis of Laplace inversions. Thus, two- and three-site kinetics models were applied to extract porosity from relaxation decays, thereby improving the utility of the porosity screening tool. (C) 2014 Elsevier Inc. All rights reserved. C1 [Chen, Joseph J.; Reimer, Jeffrey A.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Mason, Jarad A.; Bloch, Eric D.; Gygi, David; Long, Jeffrey R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Long, Jeffrey R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Chen, JJ (reprint author), Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. FU U.S. Department of Energy, Advanced Research Projects Agency - Energy (ARPA-E) [DE- AR0000103]; NSF FX The information, data, or work presented herein was funded by the U.S. Department of Energy, Advanced Research Projects Agency - Energy (ARPA-E) under Grant No. DE- AR0000103. The authors acknowledge Dr. Kenji Sumida, and Ms. Mary Anne Manumpil for assistance with sample preparation. We also thank NSF for providing graduate fellowship support for J.A.M. NR 25 TC 0 Z9 0 U1 5 U2 41 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 1387-1811 EI 1873-3093 J9 MICROPOR MESOPOR MAT JI Microporous Mesoporous Mat. PD MAR 15 PY 2015 VL 205 SI SI BP 65 EP 69 DI 10.1016/j.micromeso.2014.07.037 PG 5 WC Chemistry, Applied; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CC2QU UT WOS:000350190500016 ER PT J AU Lim, YC Squires, L Pan, TY Miles, M Song, GL Wang, YL Feng, ZL AF Lim, Yong Chae Squires, Lile Pan, Tsung-Yu Miles, Michael Song, Guang-Ling Wang, Yanli Feng, Zhili TI Study of mechanical joint strength of aluminum alloy 7075-T6 and dual phase steel 980 welded by friction bit joining and weld-bonding under corrosion medium SO MATERIALS & DESIGN LA English DT Article DE Dissimilar material joining; Aluminum alloy; Dual phase steel; Friction bit joining; Mechanical properties; Corrosion ID NACL SOLUTION; GALVANIC CORROSION; DISSIMILAR JOINTS; MAGNESIUM ALLOYS; MICROSTRUCTURE; BEHAVIOR; IRON AB In this work, we have employed a unique solid-sate joining process, called friction bit joining (FBJ), to spot weld aluminum alloy (AA) 7075-T6 and dual phase (DP) 980 steel. Static joint strength was studied in the lap shear tension configuration. In addition, weld-bonding (adhesive + FBJ) joints were studied in order to evaluate the ability of adhesive to mitigate the impact of corrosion on joint properties. Accelerated laboratory cyclic corrosion tests were carried out for both FBJ only and weld-bonding joints. The FBJ only joints that emerged from corrosion testing had lap shear failure loads that were significantly lower than freshly prepared joints. However, weld-bonding specimens retained more than 80% of the lap shear failure load of the freshly prepared weld-bonding specimens. Examination of joint cross sections confirmed that the presence of adhesive in the weld-bonding joints mitigated the effect of the corrosion environment, compared to FBJ only joints. (C) 2014 Elsevier Ltd. All rights reserved. C1 [Lim, Yong Chae; Pan, Tsung-Yu; Song, Guang-Ling; Wang, Yanli; Feng, Zhili] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Squires, Lile; Miles, Michael] Brigham Young Univ, Provo, UT 84602 USA. RP Feng, ZL (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, One Bethel Valley Rd, Oak Ridge, TN 37831 USA. EM limy@ornl.gov; lpsquires@gmail.com; pant@ornl.gov; mmiles@byu.edu; songg@ornl.gov; wangy3@ornl.gov; fengz@ornl.gov RI Feng, Zhili/H-9382-2012; Song, Guang-Ling/D-9540-2013; OI Feng, Zhili/0000-0001-6573-7933; Song, Guang-Ling/0000-0002-9802-6836; Lim, Yong Chae/0000-0003-2177-3988 FU U.S. Department of Energy, Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies, Lightweight Materials Program; U.S. Department of Energy [DE-AC05-00OR22725] FX This research was financially sponsored by the U.S. Department of Energy, Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies, as part of the Lightweight Materials Program. Oak Ridge National Laboratory (ORNL) is managed by UT-Battelle, LLC for the U.S. Department of Energy under Contract DE-AC05-00OR22725. NR 40 TC 3 Z9 3 U1 6 U2 50 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0264-1275 EI 1873-4197 J9 MATER DESIGN JI Mater. Des. PD MAR 15 PY 2015 VL 69 BP 37 EP 43 DI 10.1016/j.matdes.2014.12.043 PG 7 WC Materials Science, Multidisciplinary SC Materials Science GA CB4TD UT WOS:000349620200005 ER PT J AU Jemison, M Sussman, M Shashkov, M AF Jemison, Matthew Sussman, Mark Shashkov, Mikhail TI Filament capturing with the Multimaterial Moment-of-Fluid method SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Interface reconstruction; Moving boundary problem; Moment-of-Fluid method; Filament capturing ID INCOMPRESSIBLE 2-PHASE FLOWS; ADAPTIVE LEVEL SET; INTERFACE TRACKING; FRONT-TRACKING; RECONSTRUCTION AB A novel method for capturing two-dimensional, thin, under-resolved material configurations, known as "filaments," is presented in the context of interface reconstruction. This technique uses a partitioning procedure to detect disconnected regions of material in the advective preimage of a cell (indicative of a filament) and makes use of the existing functionality of the Multimaterial Moment-of-Fluid interface reconstruction method to accurately capture the under-resolved feature, while exactly conserving volume. An algorithm for Adaptive Mesh Refinement in the presence of filaments is developed so that refinement is introduced only near the tips of filaments and where the Moment-of-Fluid reconstruction error is still large. Comparison to the standard Moment-of-Fluid method is made. It is demonstrated that using filament capturing at a given resolution yields gains in accuracy comparable to introducing an additional level of mesh refinement at significantly lower cost. (C) 2015 Elsevier Inc. All rights reserved. C1 [Jemison, Matthew; Sussman, Mark] Florida State Univ, Dept Appl & Computat Math, Tallahassee, FL 32306 USA. [Shashkov, Mikhail] Los Alamos Natl Lab, X Computat Phys Div, Los Alamos, NM USA. RP Sussman, M (reprint author), Florida State Univ, Dept Appl & Computat Math, Tallahassee, FL 32306 USA. EM sussman@math.fsu.edu FU National Science Foundation [DMS 1016381]; U.S. Department of Energy's NNSA as part of Los Alamos National Laboratory's Computational Physics Student Summer Workshop [DE-AC52-06NA25396]; National Nuclear Security Administration of the US Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396]; DOE Advanced Simulation and Computing (ASC) program; DOE Office of Science ASCR Program FX Work supported in part by the National Science Foundation under contract DMS 1016381.; This work of M. Jemison was performed under the auspices of the U.S. Department of Energy's NNSA as part of Los Alamos National Laboratory's Computational Physics Student Summer Workshop organized by Scott Runnels. Los Alamos National Laboratory is operated by Los Alamos National Security, LLC, under contract number DE-AC52-06NA25396.; This work of M. Shashkov was performed under the auspices of the National Nuclear Security Administration of the US Department of Energy at Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396 and supported by the DOE Advanced Simulation and Computing (ASC) program. M. Shashkov also acknowledges the partial support of the DOE Office of Science ASCR Program. NR 25 TC 3 Z9 3 U1 1 U2 7 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD MAR 15 PY 2015 VL 285 BP 149 EP 172 DI 10.1016/j.jcp.2015.01.014 PG 24 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA CB4LP UT WOS:000349599500011 ER PT J AU Thompson, AP Swiler, LP Trott, CR Foiles, SM Tucker, GJ AF Thompson, A. P. Swiler, L. P. Trott, C. R. Foiles, S. M. Tucker, G. J. TI Spectral neighbor analysis method for automated generation of quantum-accurate interatomic potentials SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Interatomic potential; Machine learning; Spectral neighbor analysis potential; SNAP; Gaussian approximation potentials; Molecular dynamics ID TANTALUM; MOLYBDENUM; TUNGSTEN AB We present a new interatomic potential for solids and liquids called Spectral Neighbor Analysis Potential (SNAP). The SNAP potential has a very general form and uses machine-learning techniques to reproduce the energies, forces, and stress tensors of a large set of small configurations of atoms, which are obtained using high-accuracy quantum electronic structure (QM) calculations. The local environment of each atom is characterized by a set of bispectrum components of the local neighbor density projected onto a basis of hyperspherical harmonics in four dimensions. The bispectrum components are the same bond-orientational order parameters employed by the GAP potential[1]. The SNAP potential, unlike GAP, assumes a linear relationship between atom energy and bispectrum components. The linear SNAP coefficients are determined using weighted least-squares linear regression against the full QM training set. This allows the SNAP potential to be fit in a robust, automated manner to large QM data sets using many bispectrum components. The calculation of the bispectrum components and the SNAP potential are implemented in the LAMMPS parallel molecular dynamics code. We demonstrate that a previously unnoticed symmetry property can be exploited to reduce the computational cost of the force calculations by more than one order of magnitude. We present results for a SNAP potential for tantalum, showing that it accurately reproduces a range of commonly calculated properties of both the crystalline solid and the liquid phases. In addition, unlike simpler existing potentials, SNAP correctly predicts the energy barrier for screw dislocation migration in BCC tantalum. (C) 2014 Elsevier Inc. All rights reserved. C1 [Thompson, A. P.] Sandia Natl Labs, Multiscale Sci Dept, Albuquerque, NM 87185 USA. [Swiler, L. P.] Sandia Natl Labs, Optimizat & Uncertainty Quantificat Dept, Albuquerque, NM 87185 USA. [Trott, C. R.] Sandia Natl Labs, Scalable Algorithms Dept, Albuquerque, NM 87185 USA. [Foiles, S. M.; Tucker, G. J.] Sandia Natl Labs, Computat Mat & Data Sci Dept, Albuquerque, NM 87185 USA. [Tucker, G. J.] Drexel Univ, Dept Mat Sci & Engn, Philadelphia, PA 19104 USA. RP Thompson, AP (reprint author), Sandia Natl Labs, Multiscale Sci Dept, POB 5800,MS 1322, Albuquerque, NM 87185 USA. EM athomps@sandia.gov; lpswile@sandia.gov; crtrott@sandia.gov; foiles@sandia.gov; gtucker@coe.drexel.edu RI Tucker, Garritt/A-1954-2016; OI Tucker, Garritt/0000-0002-4011-450X; Foiles, Stephen/0000-0002-1907-454X FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors acknowledge helpful discussions with Stan Moore and Jonathan Moussa on the symmetry properties of bispectrum components. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 28 TC 12 Z9 12 U1 2 U2 26 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD MAR 15 PY 2015 VL 285 BP 316 EP 330 DI 10.1016/j.jcp.2014.12.018 PG 15 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA CB4LP UT WOS:000349599500019 ER PT J AU Zhou, HY Attard, TL Dhiradhamvit, K Wang, YL Erdman, D AF Zhou, Hongyu Attard, Thomas L. Dhiradhamvit, Kittinan Wang, Yanli Erdman, Donald TI Crashworthiness characteristics of a carbon fiber reinforced dual-phase epoxy-polyurea hybrid matrix composite SO COMPOSITES PART B-ENGINEERING LA English DT Article DE Polymer matrix composites (PMCs); Hybrid; Impact behavior; Damage tolerance; Polyurea ID ENERGY-ABSORPTION; SQUARE TUBES; REHABILITATION; PERFORMANCE; STRENGTH; POLYMER AB The crashworthiness characteristics of rectangular tubes made from a Carbon-fiber reinforced Hybrid-Polymeric Matrix (CHMC) composite were investigated using quasi-static and impact crush tests. The hybrid matrix formulation of the CHMC was created by combining an epoxy-based thermosetting polymer with a lightly crosslinked polyurea elastomer at various cure-time intervals and volumetric ratios. The load displacement responses of both CHMC and carbon-fiber reinforced epoxy (CF/epoxy) specimens were obtained under various crushing speeds; and crashworthiness parameters, such as the average crushing force and specific energy absorption (SEA), were calculated using subsequent load displacement relationships. The CHMC maintained a high level of structural integrity and post-crush performance, relative to traditional CF/epoxy. The influence of the curing time and volumetric ratios of the polyurea/epoxy dual-hybridized matrix system on the crashworthiness parameters was also investigated. The results reveal that the load carrying capacity and total energy absorption tend to increase with greater polyurea thickness and lower elapsed reaction curing time of the epoxy although this is typically a function of the loading rate. Finally, the mechanism by which the CHMC provides increased damage tolerance was also investigated using scanning electron microscopy (SEM). (C) 2014 Elsevier Ltd. All rights reserved. C1 [Zhou, Hongyu] Univ Alabama, Huntsville, AL 35899 USA. [Attard, Thomas L.; Dhiradhamvit, Kittinan] Univ Alabama Birmingham, Birmingham, AL 35294 USA. [Wang, Yanli; Erdman, Donald] Oak Ridge Natl Lab, Mech Properties & Mech Grp, Oak Ridge, TN 37831 USA. RP Zhou, HY (reprint author), 5000 Tech Dr, Huntsville, AL USA. EM hongyu.zhou@uah.edu FU Department of Homeland Security through the Higher Education Research Experience (HERE) Program; Southeast Region Research Initiative (SERRI) at the Department of Energy's Oak Ridge National Laboratory (ORNL), DHS Project [90300]; U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Vehicle Technologies Program FX This research was partially supported by the Department of Homeland Security through the Higher Education Research Experience (HERE) Program, and the Southeast Region Research Initiative (SERRI) at the Department of Energy's Oak Ridge National Laboratory (ORNL), DHS Project No. 90300. This research through the Oak Ridge National Laboratory's High Temperature Materials Laboratory User Program was sponsored by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Vehicle Technologies Program. NR 33 TC 4 Z9 4 U1 3 U2 33 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 1359-8368 EI 1879-1069 J9 COMPOS PART B-ENG JI Compos. Pt. B-Eng. PD MAR 15 PY 2015 VL 71 BP 17 EP 27 DI 10.1016/j.compositesb.2014.10.053 PG 11 WC Engineering, Multidisciplinary; Materials Science, Composites SC Engineering; Materials Science GA CA4QG UT WOS:000348889100003 ER PT J AU Anderson, R Bridges, JC Williams, A Edgar, L Ollila, A Williams, J Nachon, M Mangold, N Fisk, M Schieber, J Gupta, S Dromart, G Wiens, R Le Mouelic, S Forni, O Lanza, N Mezzacappa, A Sautter, V Blaney, D Clark, B Clegg, S Gasnault, O Lasue, J Leveille, R Lewin, E Lewis, KW Maurice, S Newsom, H Schwenzer, SP Vaniman, D AF Anderson, Ryan Bridges, J. C. Williams, A. Edgar, L. Ollila, A. Williams, J. Nachon, M. Mangold, N. Fisk, M. Schieber, J. Gupta, S. Dromart, G. Wiens, R. Le Mouelic, S. Forni, O. Lanza, N. Mezzacappa, A. Sautter, V. Blaney, D. Clark, B. Clegg, S. Gasnault, O. Lasue, J. Leveille, R. Lewin, E. Lewis, K. W. Maurice, S. Newsom, H. Schwenzer, S. P. Vaniman, D. TI ChemCam results from the Shaler outcrop in Gale crater, Mars SO ICARUS LA English DT Article DE Mars; Mars, surface; Mineralogy; Spectroscopy ID INDUCED BREAKDOWN SPECTROSCOPY; INSTRUMENT SUITE; DISTANCES; METEORITE; CHLORINE; SULFUR; UNIT AB The ChemCam campaign at the fluvial sedimentary outcrop "Shaler" resulted in observations of 28 non-soil targets, 26 of which included active laser induced breakdown spectroscopy (LIBS), and all of which included Remote Micro-Imager (RMI) images. The Shaler outcrop can be divided into seven facies based on gain size, texture, color, resistance to erosion, and sedimentary structures. The ChemCam observations cover Facies 3 through 7. For all targets, the majority of the grains were below the limit of the RMI resolution, but many targets had a portion of resolvable grains coarser than similar to 0.5 mm. The Shaler facies show significant scatter in LIBS spectra and compositions from point to point, but several key compositional trends are apparent, most notably in the average K2O content of the observed facies. Facies 3 is lower in K2O than the other facies and is similar in composition to the "snake," a clastic dike that occurs lower in the Yellowknife Bay stratigraphic section. Facies 7 is enriched in 1(20 relative to the other fades and shows some compositional and textural similarities to float rocks near Yellowknife Bay. The remaining facies (4, 5, and 6) are similar in composition to the Sheepbed and Gillespie Lake members, although the Shaler fades have slightly elevated K2O and FeOT. Several analysis points within Shaler suggest the presence of feldspars, though these points have excess FeOT which suggests the presence of Fe oxide cement or inclusions. The majority of LIBS analyses have compositions which indicate that they are mixtures of pyroxene and feldspar. The Shaler feldspathic compositions are more alkaline than typical feldspars from shergottites, suggesting an alkaline basaltic source region, particularly for the K2O enriched Facies 7. Apart from possible iron-oxide cement, there is little evidence for chemical alteration at Shaler, although calcium-sulfate veins comparable to those observed lower in the stratigraphic section are present. The differing compositions, and inferred provenances at Shaler, suggest compositionally heterogeneous terrain in the Gale crater rim and surroundings, and intermittent periods of deposition. Published by Elsevier Inc. C1 [Anderson, Ryan] US Geol Survey, Astrogeol Sci Ctr, Flagstaff, AZ 86001 USA. [Bridges, J. C.] Univ Leicester, Space Res Ctr, Dept Phys & Astron, Leicester LE1 7RH, Leics, England. [Williams, A.] Univ Calif Davis, Dept Earth & Planetary Sci, Davis, CA 95616 USA. [Edgar, L.] Arizona State Univ, Sch Earth & Space Explorat, Tempe, AZ 85287 USA. [Ollila, A.; Williams, J.; Newsom, H.] Univ New Mexico, Dept Earth & Planetary Sci, Albuquerque, NM 87131 USA. [Nachon, M.; Mangold, N.; Le Mouelic, S.] Univ Nantes, CNRS, Lab Planetol & Geodynam Nantes, F-44322 Nantes, France. [Fisk, M.] Oregon State Univ, Coll Earth Ocean & Atmospher Sci, Corvallis, OR 97331 USA. [Schieber, J.] Indiana Univ, Dept Geol Sci, Bloomington, IN 47405 USA. [Gupta, S.] Univ London Imperial Coll Sci Technol & Med, Dept Earth Sci & Engn, London SW7 2AZ, England. [Dromart, G.] Univ Lyon, Lab Geol Lyon, F-69364 Lyon, France. [Lanza, N.; Clegg, S.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Forni, O.; Gasnault, O.; Lasue, J.; Maurice, S.] CNRS, IRAP, F-31028 Toulouse 4, France. [Forni, O.; Gasnault, O.; Lasue, J.; Maurice, S.] Univ Toulouse, UPS OMP, IRAP, Toulouse, France. [Mezzacappa, A.] Delaware State Univ, Optic Sci Ctr Appl Res, Dover, DE 19901 USA. [Sautter, V.] Museum Hist Nat Paris, F-75005 Paris, France. [Blaney, D.] NASA, Jet Prop Lab, Pasadena, CA 91109 USA. [Clark, B.] Space Sci Inst, Boulder, CO 80301 USA. [Leveille, R.] McGill Univ, Dept Nat Resource Sci, Ste Anne De Bellevue, PQ H9X 3V9, Canada. [Lewin, E.] Univ Grenoble 1, ISTerre, Grenoble, France. [Lewis, K. W.] Johns Hopkins Univ, Baltimore, MD 21218 USA. [Schwenzer, S. P.] Open Univ, Dept Phys Sci, Milton Keynes LE1 7RH, Bucks, England. [Vaniman, D.] Planetary Sci Inst, Tucson, AZ 85719 USA. RP Anderson, R (reprint author), US Geol Survey, Astrogeol Sci Ctr, 2255 N Gemini Dr, Flagstaff, AZ 86001 USA. EM rbanderson@usgs.gov; jcb36@leicester.ac.uk; amywill@ucdavis.edu; ledgarl@asu.edu; aollila@unm.edu; josh505@unm.edu; marion.nach@gmail.com; nicolas.mangold@univ-nantes.fr; Martin.Fisk@oregonstate.edu; jschiebe@indiana.edu; s.gupta@imperial.ac.uk; gilles.dromart@ens-Iyon.fr; rwiens@lanl.gov; stephane.lemouelic@univ-nantes.fr; olivier.forni@irap.omp.eu; nlanza@lanl.gov; amezzacappa09@students.desu.edu; vsautter@mnhn.fr; diana.Lblaney@jpl.nasa.gov; bclark@spacescience.org; sclegg@lanl.gov; olivier.gasnault@irap.omp.eu; jeremie.lasue@irap.omp.eu; rich.leveille@gmail.com; Eric.LEWIN@obs.ujf-grenoble.fr; sylvestre.maurice@irap.omp.eu; newsom@unm.edu; dvaniman@psi.edu RI Williams, Amy/B-6623-2014; LEWIN, Eric/F-1451-2017; OI Williams, Amy/0000-0001-6299-0845; Gasnault, Olivier/0000-0002-6979-9012; Schwenzer, Susanne Petra/0000-0002-9608-0759; Clegg, Sam/0000-0002-0338-0948 FU Mars Science Laboratory project; Centre National d'Etudes Spatiales (CNES); Shoemaker Postdoctoral Fellowship; UK Space Agency; National Aeronautics and Space Administration FX This work was supported by the Mars Science Laboratory project. The French contribution to ChemCam on MSL is supported by the Centre National d'Etudes Spatiales (CNES). Anderson acknowledges support from the Shoemaker Postdoctoral Fellowship. Gupta, Bridges, and Schwenzer acknowledge the support of the UK Space Agency. Contributions from Blaney have been conducted at the Jet Propulsion Laboratory, California Institute of Technology under a contract with the National Aeronautics and Space Administration. We thank Brian Balta and an anonymous reviewer for their thoughtful and constructive comments. NR 49 TC 10 Z9 10 U1 7 U2 57 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0019-1035 EI 1090-2643 J9 ICARUS JI Icarus PD MAR 15 PY 2015 VL 249 SI SI BP 2 EP 21 DI 10.1016/j.icarus.2014.07.025 PG 20 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CA5SE UT WOS:000348967300002 ER PT J AU Cousin, A Meslin, PY Wiens, RC Rapin, W Mangold, N Fabre, C Gasnault, O Forni, O Tokar, R Ollila, A Schroder, S Lasue, J Maurice, S Sautter, V Newsom, H Vaniman, D Le Mouelic, S Dyar, D Berger, G Blaney, D Nachon, M Dromart, G Lanza, N Clark, B Clegg, S Goetz, W Berger, J Barraclough, B Delapp, D AF Cousin, A. Meslin, P. Y. Wiens, R. C. Rapin, W. Mangold, N. Fabre, C. Gasnault, O. Forni, O. Tokar, R. Ollila, A. Schroeder, S. Lasue, J. Maurice, S. Sautter, V. Newsom, H. Vaniman, D. Le Mouelic, S. Dyar, D. Berger, G. Blaney, D. Nachon, M. Dromart, G. Lanza, N. Clark, B. Clegg, S. Goetz, W. Berger, J. Barraclough, B. Delapp, D. CA MSL Sci Team TI Compositions of coarse and fine particles in martian soils at gale: A window into the production of soils SO ICARUS LA English DT Article DE Mars; Mars, surface; Spectroscopy; Regoliths ID INDUCED BREAKDOWN SPECTROSCOPY; CHEMCAM INSTRUMENT SUITE; CHEMICAL-COMPOSITION; MARS; LASER; ROVER; PATHFINDER; CHEMISTRY; TARGETS; ROCKS AB The ChemCam instrument onboard the Curiosity rover provides for the first time an opportunity to study martian soils at a sub-millimeter resolution. In this work, we analyzed 24 soil targets probed by ChemCam during the first 250 sols on Mars. Using the depth profile capability of the ChemCam LIBS (Laser-Induced Breakdown Spectroscopy) technique, we found that 45% of the soils contained coarse grains (>500 mu m). Three distinct clusters have been detected: Cluster 1 shows a low SiO2 content; Cluster 2 corresponds to coarse grains with a felsic composition, whereas Cluster 3 presents a typical basaltic composition. Coarse grains from Cluster 2 have been mostly observed exposed in the vicinity of the landing site, whereas coarse grains from Clusters 1 and 3 have been detected mostly buried, and were found all along the rover traverse. The possible origin of these coarse grains was investigated. Felsic (Cluster 2) coarse grains have the same origin as the felsic rocks encountered near the landing site, whereas the origin of the coarse grains from Clusters I and 3 seems to be more global. Fine-grained soils (particle size < laser beam diameter which is between 300 and 500 mu m) show a homogeneous composition all along the traverse, different from the composition of the rocks encountered at Gale. Although they contain a certain amount of hydrated amorphous component depleted in Si02, possibly present as a surface coating, their overall chemical homogeneity and their close-to-basaltic composition suggest limited, or isochemical alteration, and a limited interaction with liquid water. Fine particles and coarse grains from Cluster 1 have a similar composition, and the former could derive from weathering of the latter. Overall martian soils have a bulk composition between that of fine particles and coarse grains. This work shows that the ChemCam instrument provides a means to study the variability of soil composition at a scale not achievable by bulk chemical analyses. (C) 2014 Elsevier Inc. All rights reserved. C1 [Cousin, A.; Wiens, R. C.; Lanza, N.; Clegg, S.; Delapp, D.] Los Alamos Natl Lab, Los Alamos, NM 87544 USA. [Meslin, P. Y.; Rapin, W.; Gasnault, O.; Forni, O.; Schroeder, S.; Lasue, J.; Maurice, S.; Berger, G.] Inst Rech Astrophys & Planetol, Toulouse, France. [Mangold, N.; Le Mouelic, S.; Nachon, M.] Univ Nantes, LPGNantes, Lab Planetol & Geodynam, CNRS UMR 6112, F-44035 Nantes, France. [Fabre, C.] Univ Lorraine, Nancy, France. [Tokar, R.; Vaniman, D.; Barraclough, B.] Planetary Sci Inst, Tucson, AZ 85719 USA. [Ollila, A.; Newsom, H.] Univ New Mexico, Albuquerque, NM 87131 USA. [Sautter, V.] Museum Natl Hist Nat, F-75231 Paris, France. [Dyar, D.] Mt Holyoke Coll, S Hadley, MA 01075 USA. [Blaney, D.] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Dromart, G.] Lab Geol Lyon, Lyon, France. [Clark, B.] Space Sci Inst, Bouler, CO 80301 USA. [Goetz, W.] Max Planck Inst Solar Syst Res, Katlenburg Lindau, Germany. [Berger, J.] Western Univ, Dept Earth Sci, London, ON N6A 5B7, Canada. RP Cousin, A (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87544 USA. EM acousin@lanl.gov RI Gonzalez, Rafael/D-1748-2009; Rodriguez-Manfredi, Jose/L-8001-2014; BERGER, Gilles/F-7118-2016; Ramos, Miguel/K-2230-2014; OI Rodriguez-Manfredi, Jose/0000-0003-0461-9815; Ramos, Miguel/0000-0003-3648-6818; Gasnault, Olivier/0000-0002-6979-9012; Clegg, Sam/0000-0002-0338-0948 FU NASA's Mars Program Office FX NASA's Mars Program Office sponsored this research. The whole team acknowledges JPL for developing and leading this successful mission. The team also acknowledges CNES for its important role shared in the ChemCam operations. The data reported in this paper are archived at the Planetary Data System, accessible at http://pdsgeosciences.wustl.edu/missions/msl/index.htm. NR 73 TC 22 Z9 22 U1 4 U2 59 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0019-1035 EI 1090-2643 J9 ICARUS JI Icarus PD MAR 15 PY 2015 VL 249 SI SI BP 22 EP 42 DI 10.1016/j.icarus.2014.04.052 PG 21 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CA5SE UT WOS:000348967300003 ER PT J AU Schroder, S Meslin, PY Gasnault, O Maurice, S Cousin, A Wiens, RC Rapin, W Dyar, MD Mangold, N Forni, O Nachon, M Clegg, S Johnson, JR Lasue, J Le Mouelic, S Ollila, A Pinet, P Sautter, V Vaniman, D AF Schroeder, S. Meslin, P. -Y. Gasnault, O. Maurice, S. Cousin, A. Wiens, R. C. Rapin, W. Dyar, M. D. Mangold, N. Forni, O. Nachon, M. Clegg, S. Johnson, J. R. Lasue, J. Le Mouelic, S. Ollila, A. Pinet, P. Sautter, V. Vaniman, D. TI Hydrogen detection with ChemCam at Gale crater SO ICARUS LA English DT Article DE Mars; Mars, surface; Mineralogy; Spectroscopy ID INDUCED BREAKDOWN SPECTROSCOPY; MULTIVARIATE-ANALYSIS METHODS; INSTRUMENT SUITE; LANDING SITE; MARS; WATER; EMISSION; ROVER; CYCLE; IDENTIFICATION AB One of the main advantages of ChemCam's LIBS (Laser-Induced Breakdown Spectroscopy) instrument onboard the Curiosity rover is its potential to detect light elements such as hydrogen at fine scales, which has never been achieved on Mars. Hydrogen lines are detected in most of the data obtained within the first 320 sols of the mission at Gale crater, Mars. This work is a description of the hydrogen signal and its variability in the ChemCam LIBS spectra; it discusses the challenges of qualitative and quantitative analysis. Data acquisition and processing steps are investigated and optimized for the detection of hydrogen on Mars. Subtraction of an appropriate dark spectrum and the deconvolution of the superimposed emission of carbon from the low-pressure CO2-dominated atmosphere are particularly important. Because the intensities of hydrogen are also affected by matrix effects, the hydrogen signal was investigated within groups of targets sharing common chemical features and similar matrices. The different groups cover a variety of rock and soil compositions encountered along the traverse (calcium sulfate veins, mafic soils, felsic, Mg-rich and Fe-rich rocks) including data from both drill holes and their tailings. Almost all these targets were found to be hydrated to variable extents. Soils have systematically higher hydrogen signals than rocks and pebbles, probably as a result of their alteration. The results from rocks suggest that various alteration processes leading to their hydration have taken place, which is consistent with the fluvial lacustrine context, the diagenetic features, and the mineralogy observed by Curiosity in Yellowknife Bay. (C) 2014 Elsevier Inc. All rights reserved. C1 [Schroeder, S.; Meslin, P. -Y.; Gasnault, O.; Maurice, S.; Rapin, W.; Forni, O.; Lasue, J.; Pinet, P.] Univ Toulouse 1, UPS OMP, CNRS, IRAP, F-31028 Toulouse, France. [Cousin, A.; Wiens, R. C.; Clegg, S.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Dyar, M. D.] Mt Holyoke Coll, Dept Astron, S Hadley, MA 01075 USA. [Mangold, N.; Nachon, M.; Le Mouelic, S.] Univ Nantes, CNRS, LPGN, UMR6112, F-44322 Nantes, France. [Johnson, J. R.] Johns Hopkins Univ, Appl Phys Lab, Laurel, MD 20723 USA. [Ollila, A.] Univ New Mexico, Inst Meteorit, Dept Earth & Planetary Sci, Albuquerque, NM 87131 USA. [Sautter, V.] Museum Natl Hist Nat, F-75005 Paris, France. [Vaniman, D.] Planetary Sci Inst, Tucson, AZ 85719 USA. RP Schroder, S (reprint author), Univ Toulouse 1, UPS OMP, CNRS, IRAP, BP 44346, F-31028 Toulouse, France. EM sschroder@irap.omp.eu RI Johnson, Jeffrey/F-3972-2015; OI Gasnault, Olivier/0000-0002-6979-9012; Clegg, Sam/0000-0002-0338-0948 FU Centre National d'Etudes Spatiales (CNES); NASA's Mars Program Office FX This work was enabled by a post-doc grant by the Centre National d'Etudes Spatiales (CNES), which also supports the French operations of the ChemCam instrument. The MSL mission is funded by NASA's Mars Program Office. The whole team acknowledges JPL for developing and leading this successful mission. We acknowledge the MAHLI team for providing us with the images used to colorize the RMI images. We thank two anonymous reviewers for their helpful comments. NR 82 TC 18 Z9 18 U1 5 U2 47 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0019-1035 EI 1090-2643 J9 ICARUS JI Icarus PD MAR 15 PY 2015 VL 249 SI SI BP 43 EP 61 DI 10.1016/j.icarus.2014.08.029 PG 19 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CA5SE UT WOS:000348967300004 ER PT J AU Lanza, NL Ollila, AM Cousin, A Wiens, RC Clegg, S Mangold, N Bridges, N Cooper, D Schmidt, M Berger, J Arvidson, R Melikechi, N Newsom, HE Tokar, R Hardgrove, C Mezzacappa, A Jackson, RS Clark, B Forni, O Maurice, S Nachon, M Anderson, RB Blank, J Deans, M Delapp, D Leveille, R McInroy, R Martinez, R Meslin, PY Pinet, P AF Lanza, Nina L. a Ollila, Ann M. b Cousin, Agnes a Wiens, Roger C. a Clegg, Samuel a Mangold, Nicolas c Bridges, Nathan d Cooper, Daniel a Schmidt, Mariek e Berger, Jeffrey f Arvidson, Raymond. g Melikechi, Noureddine h Newsom, Horton E. b Tokar, Robert i Hardgrove, Craig j Mezzacappa, Alissa h Jackson, Ryan S. b Clark, Benton k Forni, Olivier Maurice, Sylvestre m Nachon, Marion c Anderson, Ryan B. n Blank, Jennifer o Deans, Matthew p Delapp, Dorothea a Leveille, Richard q McInroy, Rhonda a Martinez, Ronald a Meslin, Pierre-Yves m Pinet, Patrick m TI Understanding the signature of rock coatings in laser-induced breakdown spectroscopy data SO ICARUS LA English DT Article DE Mars, surface; Spectroscopy; Geological processes; Experimental techniques ID ATACAMA DESERT IMPLICATIONS; CHEMCAM INSTRUMENT SUITE; GUSEV CRATER; WEATHERING RINDS; SPIRIT ROVER; VARNISH FORMATION; MARS; SEARCH; SOILS; LIFE AB Surface compositional features on rocks such as coatings and weathering rinds provide important information about past aqueous environments and water rock interactions. The search for these features represents an important aspect of the Curiosity rover mission. With its unique ability to do fine-scale chemical depth profiling, the ChemCam laser-induced breakdown spectroscopy instrument (LIBS) onboard Curiosity can be used to both identify and analyze rock surface alteration features. In this study we analyze a terrestrial manganese-rich rock varnish coating on a basalt rock in the laboratory with the ChemCam engineering model to determine the LIBS signature of a natural rock coating. Results show that there is a systematic decrease in peak heights for elements such as Mn that are abundant in the coating but not the rock. There is significant spatial variation in the relative abundance of coating elements detected by LIBS depending on where on the rock surface sampled; this is due to the variability in thickness and spatial discontinuities in the coating. Similar trends have been identified in some martian rock targets in ChemCam data, suggesting that these rocks may have coatings or weathering rinds on their surfaces. (C) 2014 Elsevier Inc. All rights reserved. C1 [Lanza, Nina L. a; Cousin, Agnes a; Wiens, Roger C. a; Clegg, Samuel a; Cooper, Daniel a; Delapp, Dorothea a; McInroy, Rhonda a; Martinez, Ronald a] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Ollila, Ann M. b; Newsom, Horton E. b; Jackson, Ryan S. b] Univ New Mexico, Dept Earth & Planetary Sci, Albuquerque, NM 87131 USA. [Mangold, Nicolas c; Nachon, Marion c] Univ Nantes, CNRS, Lab Planetol & Geodynam Nantes, UMR6112, F-44322 Nantes, France. [Bridges, Nathan d] Johns Hopkins Univ, Appl Phys Lab, Laurel, MD 20723 USA. [Schmidt, Mariek e] Brock Univ, Dept Earth Sci, St Catharines, ON L2S 3A1, Canada. [Berger, Jeffrey f] Univ Western Ontario, London, ON N6A 5B7, Canada. [Arvidson, Raymond. g] Washington Univ, Dept Earth & Planetary Sci, St Louis, MO 63130 USA. [Melikechi, Noureddine h; Mezzacappa, Alissa h] Delaware State Univ, Opt Sci Ctr Appl Res, Dover, DE 19901 USA. [Tokar, Robert i] Inst Plant Sci, Tucson, AZ 85719 USA. [Hardgrove, Craig j] Arizona State Univ, Sch Earth & Space Explorat, Tempe, AZ 85281 USA. [Clark, Benton k] Space Sci Inst, Boulder, CO 80301 USA. [Forni, Olivier; Maurice, Sylvestre m; Meslin, Pierre-Yves m; Pinet, Patrick m] Univ Toulouse, F-31000 Toulouse, France. [Forni, Olivier; Maurice, Sylvestre m; Meslin, Pierre-Yves m; Pinet, Patrick m] CNRS, IRAP, F-31028 Toulouse 4, France. [Anderson, Ryan B. n] US Geol Survey, Astrogeol Sci Ctr, Flagstaff, AZ 86001 USA. [Blank, Jennifer o] Bay Area Environm Res Inst, Sonoma, CA 95476 USA. [Deans, Matthew p] NASA, Ames Res Ctr, Moffett Field, CA 94035 USA. [Leveille, Richard q] McGill Univ, Dept Nat Resource Sci, Ste Anne De Bellevue, PQ H9X 3V9, Canada. RP Lanza, NL (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM nlanza@lanl.gov; aollila@unm.edu; rwiens@lanl.gov; sclegg@lanl.gov; nicolas.mangold@univ-nantes.fr; nathan.bridges@jhuapl.edu; dcooper@lanl.gov; mschmidt2@brocku.ca; jberge44@uwo.ca; arvidson@wunder.wustl.edu; nmelikechi@desu.edu; newsom@unm.edu; rItokar@psi.edu; chardgrove@gmail.com; amezzacappa09@students.desu.edu; rjacks04@unm.edu; bclark@spacescience.org; olivier.forni@irap.omp.eu; sylvestre.maurice@irap.omp.eu; marion.nach@gmail.com; rbanderson@usgs.gov; jgblank@gmail.com; matthew.deans@nasa.gov; ddelapp@lanl.gov; rich.leveille@gmail.com; rhondam@lanl.gov; rkmartinez@lanl.gov; pmeslin@irap.omp.edu OI Clegg, Sam/0000-0002-0338-0948 FU Mars Science Laboratory project; Centre National d'Etudes Spatiales (CNES) on the French part of the ChemCam project FX This work was supported by the Mars Science Laboratory project, with additional support from the Centre National d'Etudes Spatiales (CNES) on the French part of the ChemCam project. We wish to thank M. Spilde for assistance with the SEM and two anonymous reviewers for their very helpful comments. NR 42 TC 7 Z9 9 U1 3 U2 53 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0019-1035 EI 1090-2643 J9 ICARUS JI Icarus PD MAR 15 PY 2015 VL 249 SI SI BP 62 EP 73 DI 10.1016/j.icarus.2014.05.038 PG 12 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CA5SE UT WOS:000348967300005 ER PT J AU Johnson, JR Bell, JF Bender, S Blaney, D Cloutis, E DeFlores, L Ehlmann, B Gasnault, O Gondet, B Kinch, K Lemmon, M Le Mouelic, S Maurice, S Rice, M Wiens, RC AF Johnson, Jeffrey R. Bell, J. F., III Bender, S. Blaney, D. Cloutis, E. DeFlores, L. Ehlmann, B. Gasnault, O. Gondet, B. Kinch, K. Lemmon, M. Le Mouelic, S. Maurice, S. Rice, M. Wiens, R. C. CA MSL Sci Team TI ChemCam passive reflectance spectroscopy of surface materials at the Curiosity landing site, Mars SO ICARUS LA English DT Article DE Mars; Mars, surface; Spectroscopy ID MAGNETIC-PROPERTIES EXPERIMENTS; VISIBLE/NEAR-INFRARED SPECTRA; INSTRUMENT SUITE; GUSEV CRATER; ROVER; PATHFINDER; MINERALS; SPIRIT; DUST; OPPORTUNITY AB The spectrometers on the Mars Science Laboratory (MSL) ChemCam instrument were used in passive mode to record visible/near-infrared (400-840 nm) radiance from the martian surface. Using the onboard ChemCam calibration targets' housing as a reflectance standard, we developed methods to collect, calibrate, and reduce radiance observations to relative reflectance. Such measurements accurately reproduce the known reflectance spectra of other calibration targets on the rover, and represent the highest spatial resolution (0.65 mrad) and spectral sampling (<1 nm) visible/near-infrared reflectance spectra from a landed platform on Mars. Relative reflectance spectra of surface rocks and soils match those from orbital observations and multispectral data from the MSL Mastcam camera. Preliminary analyses of the band depths, spectral slopes, and reflectance ratios of the more than 2000 spectra taken during the first year of MSL operations demonstrate at least six spectral classes of materials distinguished by variations in ferrous and ferric components. Initial comparisons of ChemCam spectra to laboratory spectra of minerals and Mars analog materials demonstrate similarities with palagonitic soils and indications of orthopyroxene in some dark rocks. Magnesium-rich "raised ridges" tend to exhibit distinct near-infrared slopes. The ferric absorption downturn typically found for martian materials at <600 nm is greatly subdued in brushed rocks and drill tailings, consistent with their more ferrous nature. Calcium-sulfate veins exhibit the highest relative reflectances observed, but are still relatively red owing to the effects of residual dust. Such dust is overall less prominent on rocks sampled within the "blast zone" immediately surrounding the landing site. These samples were likely affected by the landing thrusters, which partially removed the ubiquitous dust coatings. Increased dust coatings on the calibration targets during the first year of the mission were documented by the ChemCam passive measurements as well. Ongoing efforts to model and correct for this dust component should improve calibration of the relative reflectance spectra. This will be useful as additional measurements are acquired during the rover's future examinations of hematite-, sulfate-, and phyllosilicate-bearing materials near the base of Mt. Sharp that are spectrally active in the 400-840 nm region. (C) 2014 Elsevier Inc. All rights reserved. C1 [Johnson, Jeffrey R.] Johns Hopkins Univ, Appl Phys Lab, Laurel, MD 20723 USA. [Bell, J. F., III] Arizona State Univ, Tempe, AZ 85287 USA. [Bender, S.] Planetary Sci Inst, Tucson, AZ 85719 USA. [Blaney, D.; DeFlores, L.] Jet Prop Lab, Pasadena, CA 91109 USA. [Cloutis, E.] Univ Winnipeg, Winnipeg, MB R3B 2E9, Canada. [Ehlmann, B.; Rice, M.] CALTECH, Pasadena, CA 91125 USA. [Gasnault, O.; Maurice, S.] Univ Toulouse, CNRS, Inst Rech Astrophys & Planetol, Toulouse, France. [Gondet, B.] Inst Astrophys Spatiale, F-91405 Orsay, France. [Kinch, K.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Lemmon, M.] Texas A&M Univ, College Stn, TX 77842 USA. [Le Mouelic, S.] Univ Nantes, Lab Planetol & Geodynam, Nantes, France. [Wiens, R. C.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Johnson, JR (reprint author), Johns Hopkins Univ, Appl Phys Lab, Johns Hopkins Rd, Laurel, MD 20723 USA. EM Jeffrey.R.Johnson@jhuapl.edu RI Kinch, Kjartan/C-5742-2015; Lemmon, Mark/E-9983-2010; Gonzalez, Rafael/D-1748-2009; Rodriguez-Manfredi, Jose/L-8001-2014; Johnson, Jeffrey/F-3972-2015; Ramos, Miguel/K-2230-2014; OI Kinch, Kjartan/0000-0002-4629-8880; Lemmon, Mark/0000-0002-4504-5136; Rodriguez-Manfredi, Jose/0000-0003-0461-9815; Ramos, Miguel/0000-0003-3648-6818; Gasnault, Olivier/0000-0002-6979-9012 FU Mars Science Laboratory Participating Scientist program; Centre National d'Etudes Spatiales (CNES); Danish Council for Independent Research/Natural Sciences (FNU) [12-127126] FX The authors wish to thank the entire engineering and science teams who were integral in landing the Curiosity rover successfully, and in operating a complicated science instrument package efficiently to maximize the science return. In particular, the diligence of the downlink and uplink teams is truly appreciated, as is the generosity of the ChemCam team in agreeing to use the instrument in a manner distinct from its main purpose. The results demonstrated the excellent sensitivity of the instrument's spectrometers and the benefits of flexibility when operating instruments on Mars. K. Seelos UHU/APL) provided the CRISM spectrum, and A. Ody (Universite Paris-Sud, Orsay, France) provided the bright and dark OMEGA spectra. S. Clegg (LANL) provided the list of ChemCam targets assigned to specific geologic units. Helpful reviews were provided by M. Lane and an anonymous reviewer. J.R. Johnson was funded by the Mars Science Laboratory Participating Scientist program. The French contribution to MSL is supported by the Centre National d'Etudes Spatiales (CNES). Work by K. Kinch was supported by the Danish Council for Independent Research/Natural Sciences (FNU Grant 12-127126). NR 71 TC 4 Z9 4 U1 5 U2 33 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0019-1035 EI 1090-2643 J9 ICARUS JI Icarus PD MAR 15 PY 2015 VL 249 SI SI BP 74 EP 92 DI 10.1016/j.icarus.2014.02.028 PG 19 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CA5SE UT WOS:000348967300006 ER PT J AU Le Mouelic, S Gasnault, O Herkenhoff, KE Bridges, NT Langevin, Y Mangold, N Maurice, S Wiens, RC Pinet, P Newsom, HE Deen, RG Bell, JF Johnson, JR Rapin, W Barraclough, B Blaney, DL Deflores, L Maki, J Malin, MC Perez, R Saccoccio, M AF Le Mouelic, S. Gasnault, O. Herkenhoff, K. E. Bridges, N. T. Langevin, Y. Mangold, N. Maurice, S. Wiens, R. C. Pinet, P. Newsom, H. E. Deen, R. G. Bell, J. F., III Johnson, J. R. Rapin, W. Barraclough, B. Blaney, D. L. Deflores, L. Maki, J. Malin, M. C. Perez, R. Saccoccio, M. TI The ChemCam Remote Micro-Imager at Gale crater: Review of the first year of operations on Mars SO ICARUS LA English DT Article DE Mars; Mars, surface; Mineralogy; Data reduction techniques; Image processing ID INSTRUMENT SUITE; CURIOSITY ROVER; SYSTEM; UNIT AB The Mars Science Laboratory rover, "Curiosity" landed near the base of a 5 km-high mound of layered material in Gale crater. Mounted on the rover mast, the ChemCam instrument is designed to remotely determine the composition of soils and rocks located a few meters from the rover, using a Laser-Induced Breakdown Spectrometer (LIBS) coupled to a Remote Micro-Imager (RMI). We provide an overview of the diverse imaging investigations that were carried out by ChemCam's RMI during the first year of operation on Mars. 1182 individual panchromatic RMI images were acquired from Sol 10 to Sol 360 to document the ChemCam LIBS measurements and to characterize soils, rocks and rover hardware. We show several types of derived imaging products, including mosaics of images taken before and after laser shots, difference images to enhance the most subtle laser pits, merges with color Mastcam-100 images, micro-topography using the Z-stack technique, and time lapse movies. The very high spatial resolution of RMI is able to resolve rock textures at sub-mm scales, which provides clues regarding the origin (igneous versus sedimentary) of rocks, and to reveal information about their diagenetic and weathering evolution. In addition to its scientific value over the range accessible by LIES (1-7 m), we also show that RMI can also serve as a powerful long distance reconnaissance tool to characterize the landscape at distances up to several kilometers from the rover. (C) 2014 Elsevier Inc. All rights reserved. C1 [Le Mouelic, S.; Mangold, N.] Univ Nantes, CNRS UMR 6112, Lab Planetol & Geodynam, LPGNantes, F-44035 Nantes 3, France. [Gasnault, O.; Maurice, S.; Pinet, P.; Rapin, W.] Univ Toulouse, UPS OMP, IRAP, Toulouse, France. [Gasnault, O.; Maurice, S.; Pinet, P.; Rapin, W.] CNRS, IRAP, F-31028 Toulouse 4, France. [Herkenhoff, K. E.] USGS Astrogeol Sci Ctr, Flagstaff, AZ 86001 USA. [Bridges, N. T.; Johnson, J. R.] Johns Hopkins Univ, Appl Phys Lab, Laurel, MD 20723 USA. [Langevin, Y.] Inst Astrophys Spatiale, Orsay, France. [Wiens, R. C.; Barraclough, B.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Newsom, H. E.] Univ New Mexico, Albuquerque, NM 87131 USA. [Deen, R. G.; Blaney, D. L.; Deflores, L.; Maki, J.] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Bell, J. F., III] Arizona State Univ, Sch Earth & Space Explorat, Tempe, AZ 85287 USA. [Malin, M. C.] Malin Space Sci Syst, San Diego, CA 92191 USA. [Perez, R.; Saccoccio, M.] CENS, Toulouse, France. Univ London Imperial Coll Sci Technol & Med, London W12 0HS, England. RP Le Mouelic, S (reprint author), Univ Nantes, CNRS, Lab Planetol & Geodynam, 2 Rue Houssiniere,BP 92208, F-44035 Nantes 3, France. EM stephane.lemouelic@univ-nantes.fr RI Johnson, Jeffrey/F-3972-2015; Bridges, Nathan/D-6341-2016; OI Gasnault, Olivier/0000-0002-6979-9012 FU Centre National d'Etudes Spatiales (CNES); NASA's Mars Program Office; National Aeronautics and Space Administration FX This research was carried out with funding from the Centre National d'Etudes Spatiales (CNES). Work in the US was carried out under contract from NASA's Mars Program Office. The work of the JPL co-authors was carried out at the Jet Propulsion Laboratory, California Institute of Technology, under a contract with the National Aeronautics and Space Administration. We thank F. Calef, K. Edgett and also two anonymous reviewers for their very constructive remarks and inputs. The authors gratefully acknowledge JPL for developing, leading and operating this successful mission. NR 32 TC 20 Z9 20 U1 6 U2 39 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0019-1035 EI 1090-2643 J9 ICARUS JI Icarus PD MAR 15 PY 2015 VL 249 SI SI BP 93 EP 107 DI 10.1016/j.icarus.2014.05.030 PG 15 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CA5SE UT WOS:000348967300007 ER PT J AU Newsom, HE Mangold, N Kah, LC Williams, JM Arvidson, RE Stein, N Ollila, AM Bridges, JC Schwenzer, SP King, PL Grant, JA Pinet, P Bridges, NT Calef, F Wiens, RC Spray, JG Vaniman, DT Elston, WE Berger, JA Garvin, JB Palucis, MC AF Newsom, Horton E. Mangold, Nicolas Kah, Linda C. Williams, Joshua M. Arvidson, Ray E. Stein, Nathan Ollila, Ann M. Bridges, John C. Schwenzer, Susanne P. King, Penelope L. Grant, John A. Pinet, Patrick Bridges, Nathan T. Calef, Fred, III Wiens, Roger C. Spray, John G. Vaniman, David T. Elston, Wolf E. Berger, Jeff A. Garvin, James B. Palucis, Marisa C. CA MSL Sci Team TI Gale crater and impact processes - Curiosity's first 364 Sols on Mars SO ICARUS LA English DT Article DE Mars, surface; Impact processes; Cratering ID CRETACEOUS-TERTIARY BOUNDARY; YAXCOPOIL-1 DRILL CORE; CLAY MINERAL FORMATION; VALLES MARINERIS; LANDING SITE; GUSEV CRATER; SCIENCE; EVOLUTION; ORIGIN; CHICXULUB AB Impact processes at all scales have been involved in the formation and subsequent evolution of Gale crater. Small impact craters in the vicinity of the Curiosity MSL landing site and rover traverse during the 364 Sols after landing have been studied both from orbit and the surface. Evidence for the effect of impacts on basement outcrops may include loose blocks of sandstone and conglomerate, and disrupted (fractured) sedimentary layers, which are not obviously displaced by erosion. Impact ejecta blankets are likely to be present, but in the absence of distinct glass or impact melt phases are difficult to distinguish from sedimentary/volcaniclastic breccia and conglomerate deposits. The occurrence of individual blocks with diverse petrological characteristics, including igneous textures, have been identified across the surface of Bradbury Rise, and some of these blocks may represent distal ejecta from larger craters in the vicinity of Gale. Distal ejecta may also occur in the form of impact spherules identified in the sediments and drift material. Possible examples of impactites in the form of shatter cones, shocked rocks, and ropy textured fragments of materials that may have been molten have been observed, but cannot be uniquely confirmed. Modification by aeolian processes of craters smaller than 40 m in diameter observed in this study, are indicated by erosion of crater rims, and infill of craters with aeolian and airfall dust deposits. Estimates for resurfacing suggest that craters less than 15 m in diameter may represent steady state between production and destruction. The smallest candidate impact crater observed is 0.6 m in diameter. The observed crater record and other data are consistent with a resurfacing rate of the order of 10 mm/Myr; considerably greater than the rate from impact cratering alone, but remarkably lower than terrestrial erosion rates. (C) 2014 Elsevier Inc. All rights reserved. C1 [Newsom, Horton E.; Williams, Joshua M.; Ollila, Ann M.; Elston, Wolf E.] Inst Meteorit, Dept Earth & Planetary Sci, Albuquerque, NM 87131 USA. [Mangold, Nicolas] Univ Nantes, CNRS, UMR 6112, LPGN, Nantes, France. [Kah, Linda C.] Univ Tennessee, Dept Earth & Planetary Sci, Knoxville, TN 37996 USA. [Arvidson, Ray E.; Stein, Nathan] Washington Univ, St Louis, MO USA. [Bridges, John C.] Univ Leicester, Dept Phys & Astron, Space Res Ctr, Leicester LE1 7RH, Leics, England. [Schwenzer, Susanne P.] Open Univ, Dept Phys Sci, Milton Keynes MK7 6AA, Bucks, England. [King, Penelope L.] Australian Natl Univ, Res Sch Earth Sci, Canberra, ACT, Australia. [King, Penelope L.] Univ Guelph, Guelph, ON N1G 2W1, Canada. [Grant, John A.] Smithsonian Inst, Natl Air & Space Museum, Ctr Earth & Planetary Studies, Washington, DC 20560 USA. [Pinet, Patrick] Univ Toulouse 3, IRAP, Toulouse, France. [Bridges, Nathan T.] Appl Phys Lab, Laurel, MD 20723 USA. [Calef, Fred, III] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Wiens, Roger C.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Spray, John G.] Univ New Brunswick, Planetary & Space Sci Ctr, Fredericton, NB E3B 5A3, Canada. [Vaniman, David T.] Planetary Sci Inst, Tucson, AZ 85719 USA. [Berger, Jeff A.] Univ Western Ontario, London, ON, Canada. [Garvin, James B.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Palucis, Marisa C.] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. RP Newsom, HE (reprint author), Inst Meteorit, Dept Earth & Planetary Sci, Albuquerque, NM 87131 USA. RI Bridges, Nathan/D-6341-2016; King, Penelope/A-1791-2011; Ramos, Miguel/K-2230-2014; Gonzalez, Rafael/D-1748-2009; Rodriguez-Manfredi, Jose/L-8001-2014 OI King, Penelope/0000-0002-8364-9168; Ramos, Miguel/0000-0003-3648-6818; Schwenzer, Susanne Petra/0000-0002-9608-0759; Rodriguez-Manfredi, Jose/0000-0003-0461-9815 FU Mars Science Laboratory Mission (NASA/JPL); JPL FX We wish to thank the dedicated team of scientists, engineers and support personnel at JPL and the author's institutions for the creation and daily operation of the marvelous tool represented by the Curiosity rover and the orbital assets which provide context and communication for the MSL mission and science. Financial support provided by the Mars Science Laboratory Mission (NASA/JPL) and other institutional support. We also greatly appreciated the comments by several reviewers of this manuscript. NR 124 TC 14 Z9 14 U1 3 U2 28 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0019-1035 EI 1090-2643 J9 ICARUS JI Icarus PD MAR 15 PY 2015 VL 249 SI SI BP 108 EP 128 DI 10.1016/j.icarus.2014.10.013 PG 21 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CA5SE UT WOS:000348967300008 ER PT J AU Zhang, YF Bai, XM Tonks, MR Biner, SB AF Zhang, Yongfeng Bai, Xian-Ming Tonks, Michael R. Biner, S. Bulent TI Formation of prismatic loops from C15 Laves phase interstitial clusters in body-centered cubic iron SO SCRIPTA MATERIALIA LA English DT Article DE C15 cluster; Prismatic loop; Transformation; Molecular dynamics ID DISLOCATION LOOPS; MOLECULAR-DYNAMICS; INTERATOMIC POTENTIALS; ALPHA-IRON; BCC IRON; ENERGY; EVOLUTION; CASCADES; MOBILITY; METALS AB This work reports the transformation of C15 Laves phase interstitial clusters to prismatic loops in body-centered cubic iron. Molecular dynamics simulations and elasticity analysis show that, within a certain size range, C15 clusters are more stable than loops, but the relative stabilities are reversed beyond this range. C15 clusters can consistently grow by absorbing interstitials at small sizes and transforming into loops later. Both < 1 0 0 > and < 1 1 1 >/2 loops may result from the transformation, revealing a new formation mechanism for < 1 0 0 > loops. (C) 2014 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Zhang, Yongfeng; Bai, Xian-Ming; Tonks, Michael R.; Biner, S. Bulent] INL, Idaho Falls, ID 83415 USA. RP Zhang, YF (reprint author), INL, Idaho Falls, ID 83415 USA. EM yongfeng.zhang@inl.gov RI Bai, Xianming/E-2376-2017 OI Bai, Xianming/0000-0002-4609-6576 FU DOE Light Water Reactor Sustainability Program FX The authors are grateful for the support of the DOE Light Water Reactor Sustainability Program. NR 31 TC 5 Z9 5 U1 4 U2 19 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6462 J9 SCRIPTA MATER JI Scr. Mater. PD MAR 15 PY 2015 VL 98 BP 5 EP 8 DI 10.1016/j.scriptamat.2014.10.033 PG 4 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA CA5RM UT WOS:000348965500002 ER PT J AU Aidhy, DS Zhang, YW Weber, WJ AF Aidhy, Dilpuneet S. Zhang, Yanwen Weber, William J. TI Radiation damage in cubic ZrO2 and yttria-stabilized zirconia from molecular dynamics simulations SO SCRIPTA MATERIALIA LA English DT Article DE YSZ; ZrO2; Radiation damage; Molecular dynamics; Defect cluster ID URANIUM-DIOXIDE; DEFECTS; UO2; PLUTONIUM AB We perform molecular dynamics simulation on cubic ZrO2 and yttria-stabilized zirconia (YSZ) to elucidate defect cluster formation resulting from radiation damage and evaluate the impact of Y dopants. Interstitial clusters composed of split-interstitial building blocks, i.e. Zr-Zr or Y-Zr were formed. Oxygen vacancies control cation defect migration; in their presence, Zr interstitials aggregate to form split interstitials, whereas in their absence Zr interstitials remain immobile, as isolated single-interstitials. Y-doping prevents interstitial cluster formation due to sequestration of oxygen vacancies. (C) 2014 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Aidhy, Dilpuneet S.; Zhang, Yanwen; Weber, William J.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Zhang, Yanwen; Weber, William J.] Univ Tennessee, Knoxville, TN 37996 USA. RP Aidhy, DS (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. EM aidhyds@ornl.gov RI Weber, William/A-4177-2008 OI Weber, William/0000-0002-9017-7365 FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Science and Engineering Division; Office of Science, U.S. Department of Energy [DEAC02-05CH11231] FX This research was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Science and Engineering Division. The computer simulations were performed at the National Energy Research Scientific Computing Center at Lawrence Berkeley National Laboratory, which is supported by the Office of Science, U.S. Department of Energy, under Contract No. DEAC02-05CH11231. NR 34 TC 6 Z9 6 U1 0 U2 49 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6462 J9 SCRIPTA MATER JI Scr. Mater. PD MAR 15 PY 2015 VL 98 BP 16 EP 19 DI 10.1016/j.scriptamat.2014.10.036 PG 4 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA CA5RM UT WOS:000348965500005 ER PT J AU Beyerlein, IJ Carpenter, JS Hunter, A Toth, LS Skrotzki, W AF Beyerlein, I. J. Carpenter, J. S. Hunter, A. Toth, L. S. Skrotzki, W. TI Nano-enabled orientation alignment via extreme shear strains SO SCRIPTA MATERIALIA LA English DT Article DE Texture; Nanocrystals; Severe plastic deformation; Palladium; Crystal plasticity ID TEXTURE EVOLUTION; NANOCRYSTALLINE MATERIALS; PLASTIC-DEFORMATION; MECHANICAL-BEHAVIOR; GRAIN-BOUNDARIES; COPPER; CU; STRESS; METALS; POLYCRYSTALS AB It was recently shown that the crystals in an already nanocrystalline alloy (Pd-10% Au) became highly oriented under extreme shearing. No such self-ordering is seen in the coarse-grained counterpart under the same conditions. Here we use phase field dislocation dynamics and polycrystalline plasticity modeling to explore the possible causes that enabled this unusual crystallographic alignment. The results suggest that full-dislocation slip and preservation of grain boundary misorientation with at least one neighbor grain can cause the highly oriented texture observed experimentally. (C) 2014 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Beyerlein, I. J.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Carpenter, J. S.] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. [Hunter, A.] Los Alamos Natl Lab, X Computat Phys Div, Los Alamos, NM 87545 USA. [Toth, L. S.] Univ Lorraine Metz, Lab Etude Microstruct & Mecan Mat LEM3, F-57045 Metz 01, France. [Skrotzki, W.] Tech Univ Dresden, Inst Strukturphys, D-01062 Dresden, Germany. RP Beyerlein, IJ (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM Irene@lanl.gov RI toth, laszlo/A-4064-2013; OI toth, laszlo/0000-0001-7598-9026; Carpenter, John/0000-0001-8821-043X FU Laboratory Directed Research and Development program [20140348ER, 20130745ECR]; French State program "Investment in the future" [ANR-11-LABX-0008-01] FX I.J.B. and J.S.C. acknowledge the support of Laboratory Directed Research and Development program award number 20140348ER. A.H. acknowledges the support of Laboratory Directed Research and Development program award number 20130745ECR. L.S.T. was supported by the French State program "Investment in the future", operated by the National Research Agency (ANR) ANR-11-LABX-0008-01, LabEx DAMAS. NR 45 TC 4 Z9 4 U1 4 U2 24 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6462 J9 SCRIPTA MATER JI Scr. Mater. PD MAR 15 PY 2015 VL 98 BP 52 EP 55 DI 10.1016/j.scriptamat.2014.10.032 PG 4 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA CA5RM UT WOS:000348965500014 ER PT J AU Trendewicz, A Braun, R Dutta, A Ziegler, J AF Trendewicz, Anna Braun, Robert Dutta, Abhijit Ziegler, Jack TI One dimensional steady-state circulating fluidized-bed reactor model for biomass fast pyrolysis (vol 133, pg 253, 2014) SO FUEL LA English DT Correction C1 [Trendewicz, Anna; Braun, Robert] Colorado Sch Mines, Golden, CO 80401 USA. [Dutta, Abhijit; Ziegler, Jack] Natl Renewable Energy Lab, Golden, CO USA. RP Braun, R (reprint author), Colorado Sch Mines, 1500 Illinois St, Golden, CO 80401 USA. EM rbraun@mines.edu NR 1 TC 2 Z9 2 U1 2 U2 22 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0016-2361 EI 1873-7153 J9 FUEL JI Fuel PD MAR 15 PY 2015 VL 144 BP 439 EP 440 DI 10.1016/j.fuel.2014.12.053 PG 2 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA AZ2AU UT WOS:000348037800049 ER PT J AU Huterer, D Kirkby, D Bean, R Connolly, A Dawson, K Dodelson, S Evrard, A Jain, B Jarvis, M Linder, E Mandelbaum, R May, M Raccanelli, A Reid, B Rozo, E Schmidt, F Sehgal, N Slosar, A van Engelen, A Wu, HY Zhao, GB AF Huterer, Dragan Kirkby, David Bean, Rachel Connolly, Andrew Dawson, Kyle Dodelson, Scott Evrard, August Jain, Bhuvnesh Jarvis, Michael Linder, Eric Mandelbaum, Rachel May, Morgan Raccanelli, Alvise Reid, Beth Rozo, Eduardo Schmidt, Fabian Sehgal, Neelima Slosar, Anze van Engelen, Alex Wu, Hao-Yi Zhao, Gongbo TI Growth of cosmic structure: Probing dark energy beyond expansion SO ASTROPARTICLE PHYSICS LA English DT Article DE Cosmology; Large-scale structure; Dark energy ID OSCILLATION SPECTROSCOPIC SURVEY; HALO MASS FUNCTION; MATTER POWER SPECTRUM; LARGE-SCALE STRUCTURE; WEAK-LENSING SURVEYS; INTRINSIC GALAXY ALIGNMENTS; REDSHIFT-SPACE DISTORTIONS; N-BODY SIMULATIONS; DIGITAL SKY SURVEY; SDSS-III AB The quantity and quality of cosmic structure observations have greatly accelerated in recent years, and further leaps forward will be facilitated by imminent projects. These will enable us to map the evolution of dark and baryonic matter density fluctuations over cosmic history. The way that these fluctuations vary over space and time is sensitive to several pieces of fundamental physics: the primordial perturbations generated by GUT-scale physics; neutrino masses and interactions; the nature of dark matter and dark energy. We focus on the last of these here: the ways that combining probes of growth with those of the cosmic expansion such as distance-redshift relations will pin down the mechanism driving the acceleration of the Universe. One way to explain the acceleration of the Universe is invoke dark energy parameterized by an equation of state w. Distance measurements provide one set of constraints on w, but dark energy also affects how rapidly structure grows; the greater the acceleration, the more suppressed the growth of structure. Upcoming surveys are therefore designed to probe w with direct observations of the distance scale and the growth of structure, each complementing the other on systematic errors and constraints on dark energy. A consistent set of results will greatly increase the reliability of the final answer. Another possibility is that there is no dark energy, but that General Relativity does not describe the laws of physics accurately on large scales. While the properties of gravity have been measured with exquisite precision at stellar system scales and densities, within our solar system and by binary pulsar systems, its properties in different environments are poorly constrained. To fully understand if General Relativity is the complete theory of gravity we must test gravity across a spectrum of scales and densities. Rapid developments in gravitational wave astronomy and numerical relativity are directed at testing gravity in the high curvature, high density regime. Cosmological evolution provides a polar opposite test bed, probing how gravity behaves in the lowest curvature, low density environments. There are a number of different implementations of astrophysically relevant modifications of gravity. Generically, the models are able to reproduce the distance measurements while at the same time altering the growth of structure. In particular, as detailed below, the Poisson equation relating over-densities to gravitational potentials is altered, and the potential that determines the geodesics of relativistic particles (such as photons) differs from the potential that determines the motion of non-relativistic particles. Upcoming surveys will exploit these differences to determine whether the acceleration of the Universe is due to dark energy or to modified gravity. To realize this potential, both wide field imaging and spectroscopic redshift surveys play crucial roles. Projects including DES, eBOSS, DESI, PFS, LSST, Euclid, and WFIRST are in line to map more than a 1000 cubic-billion-light-year volume of the Universe. These will map the cosmic structure growth rate to 1% in the redshift range 0 < z < 2, over the last 3/4 of the age of the Universe. (C) 2014 Elsevier B.V. All rights reserved. C1 [Huterer, Dragan; Evrard, August; Wu, Hao-Yi] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Kirkby, David] UC Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. [Bean, Rachel] Cornell Univ, Dept Astron, Ithaca, NY 14853 USA. [Connolly, Andrew] Univ Washington, Dept Astron, Seattle, WA 98195 USA. [Dawson, Kyle] Univ Utah, Dept Phys & Astron, Salt Lake City, UT 84112 USA. [Dodelson, Scott] Fermilab Natl Accelerator Lab, Fermilab Ctr Particle Astrophys, Batavia, IL 60510 USA. [Dodelson, Scott] Univ Chicago, Dept Astron & Astrophys, Chicago, IL 60637 USA. [Jain, Bhuvnesh; Jarvis, Michael] Univ Penn, Dept Phys & Astron, Philadelphia, PA 19104 USA. [Linder, Eric; Reid, Beth] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Mandelbaum, Rachel] Carnegie Mellon Univ, Dept Phys, Pittsburgh, PA 15213 USA. [May, Morgan; Slosar, Anze] Brookhaven Natl Lab, Upton, NY 11973 USA. [Raccanelli, Alvise] CALTECH, NASA, Jet Prop Lab, Pasadena, CA 91109 USA. [Rozo, Eduardo] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Schmidt, Fabian] Princeton Univ, Dept Astrophys Sci, Princeton, NJ 08544 USA. [Sehgal, Neelima; van Engelen, Alex] SUNY Stony Brook, Stony Brook, NY 11794 USA. [Zhao, Gongbo] Chinese Acad Sci, Natl Astron Observ, Beijing 100012, Peoples R China. [Schmidt, Fabian] Max Planck Inst Astrophys, D-85748 Garching, Germany. RP Huterer, D (reprint author), Univ Michigan, Dept Phys, 450 Church St, Ann Arbor, MI 48109 USA. EM huterer@umich.edu RI Mandelbaum, Rachel/N-8955-2014; OI Mandelbaum, Rachel/0000-0003-2271-1527; Raccanelli, Alvise/0000-0001-6726-0438; Kirkby, David/0000-0002-8828-5463; Evrard, August/0000-0002-4876-956X NR 209 TC 20 Z9 20 U1 2 U2 92 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0927-6505 EI 1873-2852 J9 ASTROPART PHYS JI Astropart Phys. PD MAR 15 PY 2015 VL 63 SI SI BP 23 EP 41 DI 10.1016/j.astropartphys.2014.07.004 PG 19 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AT3GR UT WOS:000344824400003 ER PT J AU Rhodes, J Allen, S Benson, BA Chang, T de Putter, R Dodelson, S Dore, O Honscheid, K Linder, E Menard, B Newman, J Nord, B Rozo, E Rykoff, E Vallinotto, A Weinberg, D AF Rhodes, J. Allen, S. Benson, B. A. Chang, T. de Putter, R. Dodelson, S. Dore, O. Honscheid, K. Linder, E. Menard, B. Newman, J. Nord, B. Rozo, E. Rykoff, E. Vallinotto, A. Weinberg, D. TI Exploiting cross correlations and joint analyses SO ASTROPARTICLE PHYSICS LA English DT Editorial Material DE Dark energy; Cosmology; Cross correlations ID POLE TELESCOPE SURVEY; DIGITAL SKY SURVEY; DARK-ENERGY; REDSHIFT DISTRIBUTIONS; GALAXY CLUSTERS; COSMOLOGICAL CONSTRAINTS; PHOTOMETRIC REDSHIFTS; MASS MEASUREMENTS; SELF-CALIBRATION; LENSING SURVEYS C1 [Rhodes, J.; de Putter, R.; Dore, O.] CALTECH, Jet Prop Lab, NASA, Pasadena, CA 91109 USA. [Rhodes, J.; de Putter, R.; Dore, O.] CALTECH, Pasadena, CA 91125 USA. [Allen, S.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Allen, S.; Rykoff, E.] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Dodelson, S.; Nord, B.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Dodelson, S.] Univ Chicago, Kavli Inst Cosmol Phys, Enrico Fermi Inst, Chicago, IL 60637 USA. [Dodelson, S.] Univ Chicago, Dept Astron & Astrophys, Chicago, IL 60637 USA. [Chang, T.] Acad Sinica, IAA, Taipei 10617, Taiwan. [Honscheid, K.] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. [Honscheid, K.; Weinberg, D.] Ohio State Univ, Ctr Cosmol & Astroparticle Phys, Columbus, OH 43210 USA. [Linder, E.] Univ Calif Berkeley, Berkeley Lab, Berkeley, CA 94720 USA. [Linder, E.] Univ Calif Berkeley, Berkeley Ctr Cosmol Phys, Berkeley, CA 94720 USA. [Menard, B.] Johns Hopkins Univ, Dept Phys & Astron, Baltimore, MD 21218 USA. [Menard, B.] Univ Tokyo, Inst Phys & Math Universe, Kashiwa, Chiba 2778583, Japan. [Newman, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Newman, J.] Univ Pittsburgh, PITT PACC, Pittsburgh, PA 15260 USA. [Vallinotto, A.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Vallinotto, A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Weinberg, D.] Ohio State Univ, Dept Astron, Columbus, OH 43210 USA. RP Rhodes, J (reprint author), CALTECH, Jet Prop Lab, NASA, 4800 Oak Grove Dr,MS 169-237, Pasadena, CA 91109 USA. EM jason.d.rhodes@jpl.nasa.gov NR 78 TC 0 Z9 0 U1 0 U2 12 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0927-6505 EI 1873-2852 J9 ASTROPART PHYS JI Astropart Phys. PD MAR 15 PY 2015 VL 63 SI SI BP 42 EP 54 DI 10.1016/j.astropartphys.2014.02.009 PG 13 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AT3GR UT WOS:000344824400004 ER PT J AU Abazajian, KN Arnold, K Austermann, J Benson, BA Bischoff, C Bock, J Bond, JR Borrill, J Calabrese, E Carlstrom, JE Carvalho, CS Chang, CL Chiang, HC Church, S Cooray, A 'Crawford, TM Dawson, KS Das, S Devlin, MJ Dobbs, M Dodelson, S Dore, O Dunkley, J Errard, J Fraisse, A Gallicchio, J Halverson, NW Hanany, S Hildebrandt, SR Hincks, A Hlozek, R Holder, G Holzapfel, WL Honscheid, K Hu, W Hubmayr, J Irwin, K Jones, WC Kamionkowski, M Keating, B Keisler, R Knox, L Komatsu, E Kovac, J Kuo, CL Lawrence, C Lee, AT Leitch, E Linder, E Lubin, P McMahon, J Miller, A Newburgh, L Niemack, MD Nguyen, H Nguyen, HT Page, L Pryke, C Reichardt, CL Ruhl, JE Sehgal, N Seljak, U Sievers, J Silverstein, E Slosar, A Smith, KM Spergel, D Staggs, ST Stark, A Stompor, R Vieregg, AG Wang, G Watson, S Wollack, EJ Wu, WLK Yoon, KW Zahn, O AF Abazajian, K. N. Arnold, K. Austermann, J. Benson, B. A. Bischoff, C. Bock, J. Bond, J. R. Borrill, J. Calabrese, E. Carlstrom, J. E. Carvalho, C. S. Chang, C. L. Chiang, H. C. Church, S. Cooray, A. 'Crawford, T. M. Dawson, K. S. Das, S. Devlin, M. J. Dobbs, M. Dodelson, S. Dore, O. Dunkley, J. Errard, J. Fraisse, A. Gallicchio, J. Halverson, N. W. Hanany, S. Hildebrandt, S. R. Hincks, A. Hlozek, R. Holder, G. Holzapfel, W. L. Honscheid, K. Hu, W. Hubmayr, J. Irwin, K. Jones, W. C. Kamionkowski, M. Keating, B. Keisler, R. Knox, L. Komatsu, E. Kovac, J. Kuo, C. -L. Lawrence, C. Lee, A. T. Leitch, E. Linder, E. Lubin, P. McMahon, J. Miller, A. Newburgh, L. Niemack, M. D. Nguyen, H. Nguyen, H. T. Page, L. Pryke, C. Reichardt, C. L. Ruhl, J. E. Sehgal, N. Seljak, U. Sievers, J. Silverstein, E. Slosar, A. Smith, K. M. Spergel, D. Staggs, S. T. Stark, A. Stompor, R. Vieregg, A. G. Wang, G. Watson, S. Wollack, E. J. Wu, W. L. K. Yoon, K. W. Zahn, O. TI Neutrino physics from the cosmic microwave background and large scale structure SO ASTROPARTICLE PHYSICS LA English DT Article DE Neutrinos; Cosmology; Cosmic microwave background; Large scale structure ID OSCILLATION SPECTROSCOPIC SURVEY; DIGITAL SKY SURVEY; POWER-SPECTRUM; SDSS-III; COSMOLOGICAL IMPLICATIONS; WEIGHING NEUTRINOS; GALAXIES; TELESCOPE; SYSTEMATICS; MATTER AB This is a report on the status and prospects of the quantification of neutrino properties through the cosmological neutrino background for the Cosmic Frontier of the Division of Particles and Fields Community Summer Study long-term planning exercise. Experiments planned and underway are prepared to study the cosmological neutrino background in detail via its influence on distance-redshift relations and the growth of structure. The program for the next decade described in this document, including upcoming spectroscopic galaxy surveys eBOSS and DESI and a new Stage-IV CMB polarization experiment CMB-S4, will achieve sigma(sigma m(v)) = 16 meV and sigma(N-eff)= 0.020. Such a mass measurement will produce a high significance detection of non-zero sigma m(v), whose lower bound derived from atmospheric and solar neutrino oscillation data is about 58 meV. If neutrinos have a minimal normal mass hierarchy, this measurement will definitively rule out the inverted neutrino mass hierarchy, shedding light on one of the most puzzling aspects of the Standard Model of particle physics - the origin of mass. This precise a measurement of N-eff will allow for high sensitivity to any light and dark degrees of freedom produced in the big bang and a precision test of the standard cosmological model prediction that N-eff = 3.046. (C) 2014 Elsevier B.V. All rights reserved. C1 [Abazajian, K. N.; Cooray, A.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. [Arnold, K.; Keating, B.] Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. [Austermann, J.; Halverson, N. W.] Univ Colorado, Dept Astrophys & Planetary Sci, Boulder, CO 80309 USA. [Benson, B. A.; Carlstrom, J. E.; 'Crawford, T. M.; Gallicchio, J.; Hu, W.; Keisler, R.; Vieregg, A. G.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Bischoff, C.; Kovac, J.; Stark, A.] Harvard Smithsonian Ctr Astrophys, Cambridge, MA 02138 USA. [Bock, J.; Hildebrandt, S. R.] CALTECH, Dept Phys, Pasadena, CA 91125 USA. [Bond, J. R.; Sievers, J.] Univ Toronto, Canadian Inst Theoret Astrophys, Toronto, ON M5S 3H8, Canada. [Borrill, J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Cosmol Ctr, Berkeley, CA 94720 USA. [Calabrese, E.; Dunkley, J.] Univ Oxford, Subdept Astrophys, Oxford OX1 3RH, England. [Carvalho, C. S.] Univ Lisbon, Ctr Astron & Astrofis, P-1349018 Lisbon, Portugal. [Chiang, H. C.] Univ KwaZulu Natal, Sch Math Stat & Comp Sci, Astrophys & Cosmol Res Unit, ZA-4000 Durban, South Africa. [Church, S.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Dawson, K. S.] Univ Utah, Dept Phys & Astron, Salt Lake City, UT 84112 USA. [Das, S.; Wang, G.] Argonne Natl Lab, Dept High Energy Phys, Lemont, IL 60439 USA. [Devlin, M. J.] Univ Penn, Dept Phys & Astron, Philadelphia, PA 19104 USA. [Dobbs, M.; Holder, G.] McGill Univ, Dept Phys, Montreal, PQ H3A 2T8, Canada. [Dodelson, S.; Nguyen, H.] Fermilab Natl Accelerator Lab, Fermilab Ctr Particle Astrophys, Batavia, IL 60510 USA. [Dore, O.; Lawrence, C.; Nguyen, H. T.] CALTECH, Jet Prop Lab, Pasadena, CA USA. [Errard, J.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Fraisse, A.; Jones, W. C.] Princeton Univ, Dept Phys, Princeton, NJ 08544 USA. [Hanany, S.; Pryke, C.] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Hincks, A.] Univ British Columbia, Dept Phys & Astron, Vancouver, BC V6T 1Z4, Canada. [Hlozek, R.] Princeton Univ, Dept Astrophys Sci, Princeton, NJ 08544 USA. [Holzapfel, W. L.; Lee, A. T.; Zahn, O.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Honscheid, K.; Reichardt, C. L.; Seljak, U.] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. [Hubmayr, J.] NIST, Quantum Devices Grp, Boulder, CO 80305 USA. [Irwin, K.; Kuo, C. -L.; Silverstein, E.; Wu, W. L. K.; Yoon, K. W.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Kamionkowski, M.] Johns Hopkins Univ, Dept Phys & Astron, Baltimore, MD 21218 USA. [Knox, L.] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. [Komatsu, E.] Max Planck Inst Astrophys, D-85741 Garching, Germany. [Leitch, E.] Univ Chicago, Chicago, IL 60637 USA. [Linder, E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Lubin, P.] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA. [McMahon, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Miller, A.] Columbia Univ, Columbia Astrophys Lab, New York, NY 10027 USA. [Newburgh, L.; Page, L.] Princeton Univ, Joseph Henry Labs Phys, Princeton, NJ 08544 USA. [Niemack, M. D.] Cornell Univ, Dept Phys, Ithaca, NY 14853 USA. [Ruhl, J. E.] Case Western Reserve Univ, Dept Phys, Ctr Educ & Res Cosmol & Astrophys, Cleveland, OH 44106 USA. [Sehgal, N.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Slosar, A.] Brookhaven Natl Lab, Upton, NY 11375 USA. [Smith, K. M.] Perimeter Inst Theoret Phys, Waterloo, ON N2L 2Y5, Canada. [Spergel, D.] Princeton Univ, Dept Astrophys Sci, Princeton, NJ 08544 USA. [Stompor, R.] Univ Paris Diderot, CEA Irfu, Observ Paris, Sorbonne Paris Cite,APC,CNRS IN2P3, F-75205 Paris, France. [Watson, S.] Syracuse Univ, Dept Phys, Syracuse, NY 13244 USA. [Wollack, E. J.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. RP Abazajian, KN (reprint author), Univ Calif Irvine, Dept Phys & Astron, 4129 Frederick Reines Hall, Irvine, CA 92697 USA. EM kevork@uci.edu; arnold@ucsd.edu; jason.austermann@colorado.edu; bbenson@kicp.uchicago.edu; cbischoff@cfa.harvard.edu; jjb@astro.caltech.edu; bond@cita.utoronto.edu; jdborrill@lbl.gov; erminia.calabrese@astro.ox.ac.uk; jc@kicp.uchicago.edu; cscarvalho@oal.ul.pt; clchang@kicp.uchicago.edu; cynthia@physicschick.com; schurch@stanford.edu; acooray@uci.edu; tcrawfor@kicp.uchicago.edu; kdawson@astro.utah.edu; sudeepphys@gmail.com; devlin@physics.upenn.edu; Matt.Dobbs@McGill.ca; dodelson@fnal.gov; Olivier.P.Dore@jpl.nasa.gov; j.dunkley@physics.ox.ac.uk; josquin.errard@gmail.com; afraisse@princeton.edu; gallicchio@uchicago.edu; Nils.Halverson@colorado.edu; hanany@physics.umn.edu; srh@caltech.edu; ahincks@phas.ubc.ca; rhlozek@princeton.edu; gil.holder@gmail.com; swlh@cosmology.berkeley.edu; kh@physics.osu.edu; whu@kicp.uchicago.edu; hubmayr@nist.gov; kent.irwin@nist.gov; wcjones@princeton.edu; kamion@phajhu.edu; bkeating@ucsd.edu; rkeisler@gmail.com; Ilmox@ucdavis.edu; komatsu@MPA-Garching.MPG.DE; jmkovac@cfa.harvard.edu; clkuo@stanford.edu; charles.r.lawrence@jpl.nasa.gov; adrian.lee@berkeley.edu; eml@astro.caltech.edu; evlinder@lbl.gov; lubin@cfi.deepspace.ucsb.edu; jeffmcm@umich.edu; amber@phys.columbia.edu; newburgh@princeton.edu; niemack@cornell.edu; hogann@fnal.gov; hien.t.nguyen@jpl.nasa.gov; page@princeton.edu; pryke@physics.umn.edu; cr@berkeley.edu; ruhl@case.edu; neelima.sehgal@stonybrook.edu; useljak@berkeley.edu; sievers@cita.utoronto.ca; evas@stanford.edu; anze@bnl.gov; kmsmith@perimeterinstitute.ca; dns@astro.princeton.edu; staggs@princeton.edu; aas@cfa.harvard.edu; radek@apc.univ-paris-diderot.fr; avieregg@kicp.uchicago.edu; gwang@anl.gov; gswatson@syr.edu; edward.j.wollack@nasa.gov; wIwu@stanford.edu; kiwon@stanford.edu; zahn@berkeley.edu RI Holzapfel, William/I-4836-2015; Wollack, Edward/D-4467-2012; OI Reichardt, Christian/0000-0003-2226-9169; Stark, Antony/0000-0002-2718-9996; Wollack, Edward/0000-0002-7567-4451; Kamionkowski, Marc/0000-0001-7018-2055; Sievers, Jonathan/0000-0001-6903-5074; Carvalho, C. Sofia/0000-0002-7241-9797 NR 99 TC 86 Z9 86 U1 7 U2 87 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0927-6505 EI 1873-2852 J9 ASTROPART PHYS JI Astropart Phys. PD MAR 15 PY 2015 VL 63 SI SI BP 66 EP 80 DI 10.1016/j.astropartphys.2014.05.014 PG 15 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AT3GR UT WOS:000344824400006 ER PT J AU Kim, AG Padmanabhan, N Aldering, G Allen, SW Baltay, C Cahn, RN D'Andrea, CB Dalai, N Dawson, KS Denney, KD Eisenstein, DJ Finley, DA Freedman, WL Ho, S Holz, DE Kasen, D Kent, SM Kessler, R Kuhlmann, S Linder, EV Martini, P Nugent, PE Perlmutter, S Peterson, BM Riess, AG Rubin, D Sako, M Suntzeff, NV Suzuki, N Thomas, RC Wood-Vasey, WM Woosley, SE AF Kim, A. G. Padmanabhan, N. Aldering, G. Allen, S. W. Baltay, C. Cahn, R. N. D'Andrea, C. B. Dalai, N. Dawson, K. S. Denney, K. D. Eisenstein, D. J. Finley, D. A. Freedman, W. L. Ho, S. Holz, D. E. Kasen, D. Kent, S. M. Kessler, R. Kuhlmann, S. Linder, E. V. Martini, P. Nugent, P. E. Perlmutter, S. Peterson, B. M. Riess, A. G. Rubin, D. Sako, M. Suntzeff, N. V. Suzuki, N. Thomas, R. C. Wood-Vasey, W. M. Woosley, S. E. TI Distance probes of dark energy SO ASTROPARTICLE PHYSICS LA English DT Article DE Cosmology; Distance scale; Dark energy ID BARYON ACOUSTIC-OSCILLATIONS; ACTIVE GALACTIC NUCLEI; LUMINOUS RED GALAXIES; DIGITAL SKY SURVEY; MICROWAVE BACKGROUND ANISOTROPIES; MEASURING COSMOLOGICAL PARAMETERS; NEAR-INFRARED WAVELENGTHS; SUPERNOVA LEGACY SURVEY; HUBBLE-SPACE-TELESCOPE; WAVE STANDARD SIRENS AB This document presents the results from the Distances subgroup of the Cosmic Frontier Community Planning Study (Snowmass 2013). We summarize the current state of the field as well as future prospects and challenges. In addition to the established probes using Type Ia supernovae and baryon acoustic oscillations, we also consider prospective methods based on clusters, active galactic nuclei, gravitational wave sirens and strong lensing time delays. (C) 2014 Elsevier B.V. All rights reserved. C1 [Kim, A. G.; Aldering, G.; Cahn, R. N.; Linder, E. V.; Perlmutter, S.; Rubin, D.; Suzuki, N.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Padmanabhan, N.; Baltay, C.] Yale Univ, Dept Phys, New Haven, CT 06520 USA. [Allen, S. W.] SLAC Natl Accelerator Lab, Kavli Inst Particle Astrophys & Cosmol, Menlo Pk, CA 94025 USA. [Allen, S. W.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [D'Andrea, C. B.] Univ Portsmouth, Inst Cosmol & Gravitat, Portsmouth PO1 3FX, Hants, England. [Dalai, N.] Univ Illinois, Dept Astron, Urbana, IL 61801 USA. [Dawson, K. S.; Suzuki, N.] Univ Utah, Dept Phys & Astron, Salt Lake City, UT 84112 USA. [Denney, K. D.; Martini, P.; Peterson, B. M.] Ohio State Univ, Dept Astron, Columbus, OH 43210 USA. [Denney, K. D.; Martini, P.; Peterson, B. M.] Ohio State Univ, Ctr Cosmol & Astroparticle Phys, Columbus, OH 43210 USA. [Eisenstein, D. J.] Harvard Univ, Harvard Smithsonian Ctr Astrophys, Cambridge, MA 02138 USA. [Finley, D. A.] Fermilab Natl Accelerator Lab, Particle Phys Div, Batavia, IL 60510 USA. [Freedman, W. L.] Carnegie Observ, Pasadena, CA 91101 USA. [Ho, S.] Carnegie Mellon Univ, Dept Phys, McWilliams Ctr Cosmol, Pittsburgh, PA 15213 USA. [Holz, D. E.] Univ Chicago, Enrico Fermi Inst, Dept Phys, Chicago, IL 60637 USA. [Holz, D. E.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Kasen, D.; Perlmutter, S.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Kasen, D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Kent, S. M.] Fermilab Natl Accelerator Lab, Div Comp Sci, Batavia, IL 60510 USA. [Kessler, R.] Univ Chicago, Dept Astron & Astrophys, Chicago, IL 60637 USA. [Kuhlmann, S.] Argonne Natl Lab, Lemont, IL 60439 USA. [Linder, E. V.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Martini, P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, Berkeley, CA 94720 USA. [Riess, A. G.] Johns Hopkins Univ, Dept Phys & Astron, Baltimore, MD 21218 USA. [Sako, M.] Univ Penn, Dept Phys & Astron, Philadelphia, PA 19104 USA. [Suntzeff, N. V.] Texas A&M Univ, Dept Phys & Astron, George P & Cynthia Woods Mitchell Inst Fundamenta, College Stn, TX 77843 USA. [Wood-Vasey, W. M.] Univ Pittsburgh, Pittsburgh Particle Phys Astrophys & Cosmol Ctr P, Pittsburgh, PA 15260 USA. [Woosley, S. E.] Univ Calif Santa Cruz, Dept Astron & Astrophys, Santa Cruz, CA 95064 USA. RP Kim, AG (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM agkim@lbl.gov FU United States Department of Energy [De-AC02-07CH11359]; U.S. Department of Energy, Office of High Energy Physics [DE-AC02-05CH11231]; National Science Foundation [AST-1008882, AST-1302093]; U.S. Department of Energy [DE-AC02-765F00515]; Kavli Institute for Cosmological Physics at the University of Chicago through NSF [PHY-1125897]; DOE HEP Program [DOE-HEPDE-SC00010676]; Kavli Foundation; National Science Foundation CAREER [PHY-1151836] FX FNAL is operated by Fermi Research Alliance, LLC under Contract No. De-AC02-07CH11359 with the United States Department of Energy. LBNL is supported by the U.S. Department of Energy, Office of High Energy Physics, under Contract No. DE-AC02-05CH11231. OSU acknowledges support by the National Science Foundation under the grant AST-1008882.; SWA was supported in part by the U.S. Department of Energy under contract number DE-AC02-765F00515. KDD acknowledges support by the National Science Foundation under Award No. AST-1302093. DEH acknowledges support from National Science Foundation CAREER grant PHY-1151836, and support in part by the Kavli Institute for Cosmological Physics at the University of Chicago through NSF grant PHY-1125897 and an endowment from the Kavli Foundation and its founder Fred Kavli. DK and SEW would like to thank the DOE HEP Program for support through grant DOE-HEPDE-SC00010676. NR 191 TC 5 Z9 5 U1 2 U2 28 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0927-6505 EI 1873-2852 J9 ASTROPART PHYS JI Astropart Phys. PD MAR 15 PY 2015 VL 63 SI SI BP 2 EP 22 DI 10.1016/j.astropartphys.2014.05.007 PG 21 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA AT3GR UT WOS:000344824400002 ER PT J AU Newman, JA Abate, A Abdalla, FB Allam, S Allen, SW Ansar, R Baile, S Barkhouse, WA Beers, TC Blanton, MR Brodwin, M Brownstein, JR Brunner, RJ Kind, MC Cervantes-Cota, JL Cheu, E Chisari, NE Colless, M Comparat, J Coupon, J Cunha, CE de la Macorra, A Dell'Antonio, IP Frye, BL Gawiser, EJ Gehrels, N Grady, K Hagen, A Hall, PB Hearin, AP Hildebrandt, H Hirata, CM Ho, S Honscheid, K Huterer, D Ivezic, Z Kneib, JP Kruk, JW Lahav, O Mandelbaum, R Marshall, JL Matthews, DJ Menard, B Miguel, R Moniez, M Moos, HW Moustakas, J Myers, AD Papovich, C Peacock, JA Park, C Rahman, M Rhodes, J Ricol, JS Sadeh, I Slozar, A Schmidt, SJ Stern, DK Tyson, JA von der Linden, A Wechsler, RH Wood-Vasey, WM Zentner, AR AF Newman, Jeffrey A. Abate, Alexandra Abdalla, Filipe B. Allam, Sahar Allen, Steven W. Ansar, Reza Baile, Stephen Barkhouse, Wayne A. Beers, Timothy C. Blanton, Michael R. Brodwin, Mark Brownstein, Joel R. Brunner, Robert J. Kind, Matias Carrasco Cervantes-Cota, Jorge L. Cheu, Elliott Chisari, Nora Elisa Colless, Matthew Comparat, Johan Coupon, Jean Cunha, Carlos E. de la Macorra, Axel Dell'Antonio, Ian P. Frye, Brenda L. Gawiser, Eric J. Gehrels, Neil Grady, Kevin Hagen, Alex Hall, Patrick B. Hearin, Andew P. Hildebrandt, Hendrik Hirata, Christopher M. Ho, Shirley Honscheid, Klaus Huterer, Dragan Ivezic, Zeljko Kneib, Jean-Paul Kruk, Jeffrey W. Lahav, Ofer Mandelbaum, Rachel Marshall, Jennifer L. Matthews, Daniel J. Menard, Brice Miguel, Ramon Moniez, Marc Moos, H. W. Moustakas, John Myers, Adam D. Papovich, Casey Peacock, John A. Park, Changbom Rahman, Mubdi Rhodes, Jason Ricol, Jean-Stephane Sadeh, Iftach Slozar, Anze Schmidt, Samuel J. Stern, Daniel K. Tyson, J. Anthony von der Linden, Anja Wechsler, Risa H. Wood-Vasey, W. M. Zentner, Andrew R. TI Spectroscopic needs for imaging dark energy experiments SO ASTROPARTICLE PHYSICS LA English DT Article DE Cosmology; Dark energy; Surveys ID PHOTOMETRIC REDSHIFT ERRORS; VLT DEEP SURVEY; WEAK-LENSING TOMOGRAPHY; PHOTO-Z PERFORMANCE; DIGITAL SKY SURVEY; IA SUPERNOVAE; CROSS-CORRELATIONS; COSMIC SHEAR; PRECISION COSMOLOGY; SURVEY REQUIREMENTS AB Ongoing and near-future imaging-based dark energy experiments are critically dependent upon photometric redshifts (a.k.a. photo-z's): i.e., estimates of the redshifts of objects based only on flux information obtained through broad filters. Higher-quality, lower-scatter photo-z's will result in smaller random errors on cosmological parameters; while systematic errors in photometric redshift estimates, if not constrained, may dominate all other uncertainties from these experiments. The desired optimization and calibration is dependent upon spectroscopic measurements for secure redshift information; this is the key application of galaxy spectroscopy for imaging-based dark energy experiments. Hence, to achieve their full potential, imaging-based experiments will require large sets of objects with spectroscopically-determined redshifts, for two purposes: Training: Objects with known redshift are needed to map out the relationship between object color and z (or, equivalently, to determine empirically-calibrated templates describing the rest-frame spectra of the full range of galaxies, which may be used to predict the color-z relation). The ultimate goal of training is to minimize each moment of the distribution of differences between photometric redshift estimates and the true redshifts of objects, making the relationship between them as tight as possible. The larger and more complete our "training set" of spectroscopic redshifts is, the smaller the RMS photo-z errors should be, increasing the constraining power of imaging experiments. Requirements: Spectroscopic redshift measurements for similar to 30,000 objects over >similar to 15 widely-separated regions, each at least similar to 20 arcmin in diameter, and reaching the faintest objects used in a given experiment, will likely be necessary if photometric redshifts are to be trained and calibrated with conventional techniques. Larger, more complete samples (i.e., with longer exposure times) can improve photo-z algorithms and reduce scatter further, enhancing the science return from planned experiments greatly (increasing the Dark Energy Task Force figure of merit by up to similar to 50%). Options: This spectroscopy will most efficiently be done by covering as much of the optical and near-infrared spectrum as possible at modestly high spectral resolution (lambda/Delta lambda > similar to 3000), while maximizing the telescope collecting area, field of view on the sky, and multiplexing of simultaneous spectra. The most efficient instrument for this would likely be either the proposed GMACS/MANIFEST spectrograph for the Giant Magellan Telescope or the OPTIMOS spectrograph for the European Extremely Large Telescope, depending on actual properties when built. The PFS spectrograph at Subaru would be next best and available considerably earlier, c. 2018; the proposed ngCFHT and SSST telescopes would have similar capabilities but start later. Other key options, in order of increasing total time required, are the WFOS spectrograph at TMT, MOONS at the VLT, and DESI at the Mayall 4 m telescope (or the similar 4MOST and WEAVE projects); of these, only DESI, MOONS, and PFS are expected to be available before 2020. Table 2-3 of this white paper summarizes the observation time required at each facility for strawman training samples. To attain secure redshift measurements for a high fraction of targeted objects and cover the full redshift span of future experiments, additional near-infrared spectroscopy will also be required; this is best done from space, particularly with WFIRST-2.4 and JWST. Calibration: The first several moments of redshift distributions (the mean, RMS redshift dispersion, etc.), must be known to high accuracy for cosmological constraints not to be systematics-dominated (equivalently, the moments of the distribution of differences between photometric and true redshifts could be determined instead). The ultimate goal of calibration is to characterize these moments for every subsample used in analyses - i.e., to minimize the uncertainty in their mean redshift, RMS dispersion, etc. - rather than to make the moments themselves small. Calibration may be done with the same spectroscopic dataset used for training if that dataset is extremely high in redshift completeness (i.e., no populations of galaxies to be used in analyses are systematically missed). Accurate photo-z calibration is necessary for all imaging experiments. Requirements: If extremely low levels of systematic incompleteness (> T-p) does electron-phonon scattering at an interface contribute to thermal boundary conductance. (C) 2015 AIP Publishing LLC. C1 [Giri, Ashutosh; Gaskins, John T.; Donovan, Brian F.; Szwejkowski, Chester; Hopkins, Patrick E.] Univ Virginia, Dept Mech & Aerosp Engn, Charlottesville, VA 22904 USA. [Warzoha, Ronald J.] US Naval Acad, Dept Mech Engn, Annapolis, MD 21401 USA. [Ihlefeld, Jon] Sandia Natl Labs, Albuquerque, NM 87123 USA. RP Giri, A (reprint author), Univ Virginia, Dept Mech & Aerosp Engn, Charlottesville, VA 22904 USA. EM phopkins@virginia.edu OI Warzoha, Ronald/0000-0002-5454-4551 FU Air Force Office of Scientific Research under AFOSR [FA9550-13-1-0067, FA9550-15-1-0079]; Laboratory Directed Research and Development (LDRD) program at Sandia National Laboratories; United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This material is based upon work supported by the Air Force Office of Scientific Research under AFOSR Award Nos. FA9550-13-1-0067 and FA9550-15-1-0079. This work was also supported by the Laboratory Directed Research and Development (LDRD) program at Sandia National Laboratories. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Company, for the United States Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. P.E.H and A.G gratefully acknowledge Professor D.G. Cahill for fruitful discussions. NR 66 TC 5 Z9 5 U1 4 U2 39 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAR 14 PY 2015 VL 117 IS 10 AR 105105 DI 10.1063/1.4914867 PG 9 WC Physics, Applied SC Physics GA CD9UB UT WOS:000351442900056 ER PT J AU Long, F Daymond, MR Yao, ZW Kirk, MA AF Long, Fei Daymond, Mark R. Yao, Zhongwen Kirk, Marquis A. TI Deformation mechanism study of a hot rolled Zr-2.5Nb alloy by transmission electron microscopy. II. In situ transmission electron microscopy study of deformation mechanism change of a Zr-2.5Nb alloy upon heavy ion irradiation SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID STRESS-CORROSION CRACKING; ACTIVATED SLIP SYSTEMS; ZIRCONIUM ALLOYS; NEUTRON-IRRADIATION; GLIDING DISLOCATIONS; DYNAMICS SIMULATIONS; PRISMATIC LOOPS; ZR ALLOYS; MICROSTRUCTURE; EVOLUTION AB The effect of heavy-ion irradiation on deformation mechanisms of a Zr-2.5Nb alloy was investigated by using the in situ transmission electron microscopy deformation technique. The gliding behavior of prismatic < a > dislocations has been dynamically observed before and after irradiation at room temperature and 300 degrees C. Irradiation induced loops were shown to strongly pin the gliding dislocations. Unpinning occurred while loops were incorporated into or eliminated by < a > dislocations. In the irradiated sample, loop depleted areas with a boundary parallel to the basal plane trace were found by post-mortem observation after room temperature deformation, supporting the possibility of basal channel formation in bulk neutron irradiated samples. Strong activity of pyramidal slip was also observed at both temperatures, which might be another important mechanism to induce plastic instability in irradiated zirconium alloys. Finally, {01 (1) over bar1}< 0 (1) over bar 12 > twinning was identified in the irradiated sample deformed at 300 degrees C. (C) 2015 AIP Publishing LLC. C1 [Long, Fei; Daymond, Mark R.; Yao, Zhongwen] Queens Univ, Dept Mech & Mat Engn, Kingston, ON K7L 3N6, Canada. [Kirk, Marquis A.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Daymond, MR (reprint author), Queens Univ, Dept Mech & Mat Engn, Kingston, ON K7L 3N6, Canada. EM mark.daymond@queensu.ca OI Long, Fei/0000-0002-6522-8407; Daymond, Mark/0000-0001-6242-7489 FU U.S. Department of Energy, office of Science [DE-AC02-06CH11357]; NSERC; UNENE; Nu-Tech Precision Metals under the Industrial Research Chair program in Nuclear Materials at Queen's University FX The in situ electron microscopy was conducted at the Electron Microscopy Centre for Materials Research at Argonne National Laboratory, supported by U.S. Department of Energy, office of Science and operated under Contract No. DE-AC02-06CH11357 by UChicago Argonne, LLC. We thank Mr. Pete Boldo of Argonne National Lab for his help on the ion beam facility. This work was sponsored by NSERC, UNENE, and Nu-Tech Precision Metals under the Industrial Research Chair program in Nuclear Materials at Queen's University. NR 38 TC 2 Z9 2 U1 2 U2 14 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAR 14 PY 2015 VL 117 IS 10 AR 104302 DI 10.1063/1.4913614 PG 11 WC Physics, Applied SC Physics GA CD9UB UT WOS:000351442900027 ER PT J AU Siah, SC Winkler, MT Powell, DM Johnston, SW Kanevce, A Levi, DH Buonassisi, T AF Siah, S. C. Winkler, M. T. Powell, D. M. Johnston, S. W. Kanevce, A. Levi, D. H. Buonassisi, T. TI Proof-of-concept framework to separate recombination processes in thin silicon wafers using transient free-carrier absorption spectroscopy SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID SURFACE RECOMBINATION; CRYSTALLINE SILICON; INJECTION DEPENDENCE; SI-SIO2 INTERFACE; SOLAR-CELLS; LIFETIME; VELOCITIES; BULK; LEVEL; SEMICONDUCTORS AB We present a proof-of-concept framework to independently determine the bulk Shockley-Read-Hall (SRH) lifetime and surface recombination velocity in silicon wafers self-consistently. We measure the transient decay of free-carrier absorption (FCA) using two different excitation wavelengths (1050 and 750 nm) for p-type crystalline Si (c-Si) wafers over a wide injection range and fit the FCA transients for the two excitation wavelengths in a coupled manner. In this way, we can estimate the surface recombination lifetime accurately. However, we find that the capability to uniquely measure extrinsic bulk-SRH recombination is challenging in the presence of other recombination processes and can be broadly categorized into five different regimes depending on the relative strengths of each recombination pathway. (C) 2015 AIP Publishing LLC. C1 [Siah, S. C.; Winkler, M. T.; Powell, D. M.; Buonassisi, T.] MIT, Cambridge, MA 02139 USA. [Johnston, S. W.; Kanevce, A.; Levi, D. H.] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Siah, SC (reprint author), MIT, 77 Massachusetts Ave, Cambridge, MA 02139 USA. EM sincheng@alum.mit.edu FU National Renewable Energy Laboratory as a part of the Non-Proprietary Partnering Opportunity (NPO) Program [DE-AC36-08-GO28308]; U.S. Department of Energy; DOE [DE-EE0005314]; National Science Foundation (NSF) [ECS-0335765]; DOE under NSF CA [EEC-1041895]; Singapore NRF FX This work was supported by the National Renewable Energy Laboratory as a part of the Non-Proprietary Partnering Opportunity (NPO) Program under Contract No. DE-AC36-08-GO28308 with the U.S. Department of Energy. This work was further supported by the DOE under Contract No. DE-EE0005314, and by the National Science Foundation (NSF) and the DOE under NSF CA No. EEC-1041895. S. C. Siah acknowledges the support of Singapore NRF through a graduate fellowship. Dr. Ruiying Hao of Crystal Solar is acknowledged for providing the Epi thin silicon samples. S. Castellanos and J. Hofstetter are acknowledged for help on sample preparation and optimization of the Al2O3 passivation recipe. C. B. Simmons is acknowledged for helpful discussions. Part of this work was performed in part at the Center for Nanoscale Systems, a member of the National Nanotechnology Infrastructure Network, which was supported by the NSF under No. ECS-0335765. NR 37 TC 1 Z9 1 U1 3 U2 12 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAR 14 PY 2015 VL 117 IS 10 AR 105701 DI 10.1063/1.4914160 PG 8 WC Physics, Applied SC Physics GA CD9UB UT WOS:000351442900068 ER PT J AU Bartels, L Ernst, KH Gao, HJ Thiel, PA AF Bartels, Ludwig Ernst, Karl-Heinz Gao, Hong-Jun Thiel, Patricia A. TI Preface: Special Topic on Supramolecular Self-Assembly at Surfaces SO JOURNAL OF CHEMICAL PHYSICS LA English DT Editorial Material AB Supramolecular self-assembly at surfaces is one of the most exciting and active fields in Surface Science today. Applications can take advantage of two key properties: (i) versatile pattern formation over a broad length scale and (ii) tunability of electronic structure and transport properties, as well as frontier orbital alignment. It provides a new frontier for Chemical Physics as it uniquely combines the versatility of Organic Synthesis and the Physics of Interfaces. The Journal of Chemical Physics is pleased to publish this Special Topic Issue, showcasing recent advances and new directions. (C) 2015 AIP Publishing LLC. C1 [Bartels, Ludwig] Univ Calif Riverside, Dept Chem, Riverside, CA 92521 USA. [Bartels, Ludwig] Univ Calif Riverside, Mat Sci & Engn Program, Riverside, CA 92521 USA. [Ernst, Karl-Heinz] Swiss Fed Labs Mat Sci & Technol, EMPA, CH-8600 Dubendorf, Switzerland. [Gao, Hong-Jun] Chinese Acad Sci, Inst Phys, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China. [Thiel, Patricia A.] Iowa State Univ, Ames Lab, Dept Mat Sci & Engn, Dept Chem, Ames, IA 50011 USA. RP Bartels, L (reprint author), Univ Calif Riverside, Dept Chem, Riverside, CA 92521 USA. RI Bartels, Ludwig/C-2764-2008; Ernst, Karl-Heinz/O-6128-2015 OI Ernst, Karl-Heinz/0000-0002-2077-4922 NR 0 TC 0 Z9 0 U1 4 U2 22 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAR 14 PY 2015 VL 142 IS 10 AR 101501 DI 10.1063/1.4914017 PG 1 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CD3KT UT WOS:000350978000001 PM 25770489 ER PT J AU Somayazulu, M Dera, P Smith, J Hemley, RJ AF Somayazulu, Maddury Dera, Przemyslaw Smith, Jesse Hemley, Russell J. TI Structure and stability of solid Xe(H-2)(n) SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID EQUATION-OF-STATE; DER-WAALS COMPOUND; X-RAY-DIFFRACTION; HIGH-PRESSURE; CLATHRATE FORMATION; HARD-SPHERE; XENON; HYDROGEN; MIXTURES; TEMPERATURE AB Mixtures of xenon and molecular hydrogen form a series of hexagonal, van der Waals compounds at high pressures and at 300 K. Synchrotron, x-ray, single crystal diffraction studies reveal that below 7.5 GPa, Xe(H-2)(8) crystallizes in a P ($) over bar 3m1 structure that displays pressure-induced occupancy changes of two pairs of xenon atoms located on the 2c and 2d sites (while the third pair on yet another 2c site remains fully occupied). The occupancy becomes 1 at the P ($) over bar 3m1 to R3 transition and all the xenon atoms occupy the 3d sites in the high-pressure structure. These pressure-induced changes in occupancy coincide with volume changes that maintain the average Xe:H-2 stoichiometry fixed at 1:8. The synchrotron x-ray diffraction and Raman measurements show that this unique hydrogen-bearing compound that can be synthesized at 4.2 GPa and 300 K, quenched at low temperatures to atmospheric pressure, and retained up to 90 K on subsequent warming. (C) 2015 AIP Publishing LLC. C1 [Somayazulu, Maddury; Hemley, Russell J.] Carnegie Inst Sci, Geophys Lab, Washington, DC 20015 USA. [Dera, Przemyslaw] Univ Chicago, GSECARS, Adv Photon Source, Argonne, IL 60439 USA. [Smith, Jesse] Carnegie Inst Sci, Geophys Lab, HPCAT, Adv Photon Source, Argonne, IL 60439 USA. RP Somayazulu, M (reprint author), Carnegie Inst Sci, Geophys Lab, Washington, DC 20015 USA. EM zulu@gl.ciw.edu FU DOE-BES [DE-FG02-06ER46280, DE-FG02-99ER45775, DE-AC02-06CH11357]; DOE-NNSA (CDAC) [DE-NA-000006]; DOE-NNSA [DE-NA0001974]; NSF; Carnegie Institution of Washington FX We thank S. A. Gramsch, T. A. Strobel, and an anonymous reviewer for comments on the manuscript. The study was designed and executed with support of DOE-BES (DE-FG02-06ER46280). The facilities for Raman spectroscopy as well as financial support for M.S., P.D., and J.S. were provided by DOE-NNSA (CDAC, DE-NA-000006). Portions of this work were performed at HPCAT (Sector 16), Advanced Photon Source (APS), Argonne National Laboratory. HPCAT operations are supported by DOE-NNSA under Award No. DE-NA0001974 and DOE-BES under Award No. DE-FG02-99ER45775, with instrumentation funding provided by NSF and the Carnegie Institution of Washington. APS is supported by DOE-BES, under Contract No. DE-AC02-06CH11357. NR 54 TC 4 Z9 4 U1 3 U2 23 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAR 14 PY 2015 VL 142 IS 10 AR 104503 DI 10.1063/1.4908265 PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CD3KT UT WOS:000350978000061 PM 25770547 ER PT J AU Vogel, T Gross, J Bachmann, M AF Vogel, Thomas Gross, Jonathan Bachmann, Michael TI Thermodynamics of the adsorption of flexible polymers on nanowires SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID WALLED CARBON NANOTUBES; SELF-AVOIDING WALKS; MOLECULAR-DYNAMICS SIMULATIONS; MONTE-CARLO-SIMULATION; PHASE-TRANSITIONS; 3 DIMENSIONS; TOY MODEL; SURFACE; PROTEIN; CONFORMATIONS AB Generalized-ensemble simulations enable the study of complex adsorption scenarios of a coarse-grained model polymer near an attractive nanostring, representing an ultrathin nanowire. We perform canonical and microcanonical statistical analyses to investigate structural transitions of the polymer and discuss their dependence on the temperature and on model parameters such as effective wire thickness and attraction strength. The result is a complete hyperphase diagram of the polymer phases, whose locations and stability are influenced by the effective material properties of the nanowire and the strength of the thermal fluctuations. Major structural polymer phases in the adsorbed state include compact droplets attached to or wrapping around the wire, and tubelike conformations with triangular pattern that resemble ideal boron nanotubes. The classification of the transitions is performed by microcanonical inflection-point analysis. (C) 2015 AIP Publishing LLC. C1 [Vogel, Thomas] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Gross, Jonathan] Univ Leipzig, Inst Theoret Phys, D-04009 Leipzig, Germany. [Gross, Jonathan] Univ Leipzig, Ctr Theoret Sci NTZ, D-04009 Leipzig, Germany. [Gross, Jonathan; Bachmann, Michael] Univ Georgia, Soft Matter Syst Res Grp, Ctr Simulat Phys, Athens, GA 30602 USA. [Bachmann, Michael] Univ Fed Mato Grosso, Inst Fis, BR-78060900 Cuiaba, Mato Grosso, Brazil. [Bachmann, Michael] Univ Fed Minas Gerais, Dept Fis, BR-31270901 Belo Horizonte, MG, Brazil. RP Vogel, T (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM tvogel@lanl.gov; jonathan.gross@itp.uni-leipzig.de; bachmann@smsyslab.org OI Vogel, Thomas/0000-0003-0205-3205; Gross, Jonathan/0000-0001-8068-4235 FU NSF [DMR-1207437]; CNPq (National Council for Scientific and Technological Development, Brazil) [402091/2012-4]; DFG (German Research Foundation) [SFB/TRR 102]; Julich/Aachen/Haifa Umbrella program [SIM6, HPC_2]; Forschungszentrum Julich [jiff39, jiff43]; Georgia Advanced Computing Resource Center (GACRC) at the University of Georgia [LA-UR-14-27917] FX This work has been supported partially by the NSF under Grant No. DMR-1207437, by CNPq (National Council for Scientific and Technological Development, Brazil) under Grant No. 402091/2012-4, and by the DFG (German Research Foundation) under Grant No. SFB/TRR 102 (Project No. B04). The authors also acknowledge support by the Julich/Aachen/Haifa Umbrella program under Grant Nos. SIM6 and HPC_2. Computer time was provided by the Forschungszentrum Julich under Project Nos. jiff39 and jiff43, and by the Georgia Advanced Computing Resource Center (GACRC) at the University of Georgia. Assigned: LA-UR-14-27917. NR 76 TC 4 Z9 4 U1 7 U2 24 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAR 14 PY 2015 VL 142 IS 10 AR 104901 DI 10.1063/1.4913959 PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CD3KT UT WOS:000350978000073 PM 25770559 ER PT J AU Zhou, J Li, Y Zahl, P Sutter, P Stacchiola, DJ White, MG AF Zhou, Jing Li, Yan Zahl, Percy Sutter, Peter Stacchiola, Dario J. White, Michael G. TI Characterization of one-dimensional molecular chains of 4,4 '-biphenyl diisocyanide on Au(111) by scanning tunneling microscopy SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID SELF-ASSEMBLED MONOLAYERS; AROMATIC ISOCYANIDES; SURFACE-DEFECTS; TERMINAL GROUPS; ADSORPTION; INTERFACE; JUNCTIONS; CONDUCTION; DISPERSION; GOLD AB The morphology and electronic structure of vapor deposited 4,4'-biphenyldiisocyanide (BPDI) on a Au(111) surface were investigated using variable-temperature scanning tunneling microscopy. When deposited at room temperature, BPDI molecules form one-dimensional molecular chains similar to that recently observed for the structurally related 1,4-phenyl diisocyanide (PDI). Compared to PDI, the longer periodicity for the BPDI molecular chains is consistent with the addition of a second phenyl ring and supports a structural model in which the BPDI molecules lie parallel to the surface and interconnected by Au-adatoms. The molecular chains are mostly aligned along the [1 (1) over bar0] direction of the Au(111) substrate, but exhibit frequent changes in angle that are consistent with directions between fcc and hcp three-fold hollow sites. Dispersion-corrected density functional theory calculations for one-dimensional chains of BPDI molecules bound end-to-end via their isocyanide groups to Au-adatoms reproduce the observed periodicity of the chains and show that this morphology is energetically favored over upright binding with one free -NC group. The spatially resolved conductance (dI/dV) map for BPDI on Au(111) exhibits a feature centered at -0.67 eV below the Fermi level which are delocalized along the chain with maxima at the Au-adatom and biphenyl positions. This occupied resonant feature is close to that previously observed for the PDI in both photoemission and conductance measurements and is attributed to an occupied interfacial state resulting from BPDI-Au interactions. (C) 2015 AIP Publishing LLC. C1 [Zhou, Jing; White, Michael G.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Li, Yan] Brookhaven Natl Lab, Computat Sci Ctr, Upton, NY 11973 USA. [Zahl, Percy; Sutter, Peter] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Stacchiola, Dario J.; White, Michael G.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. RP Zhou, J (reprint author), Appl Mat Inc, Santa Clara, CA 95054 USA. RI Stacchiola, Dario/B-1918-2009 OI Stacchiola, Dario/0000-0001-5494-3205 FU U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10086, DE-AC02-98CH10886] FX The authors would like to thank Sally Swanson (IBM) for providing the BPDI sample. Work performed by J.Z. and M.G.W. in the Chemistry Department at Brookhaven National Laboratory was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10086. STM measurements and calculations were carried out at the Center for Functional Nanomaterials at Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. NR 43 TC 2 Z9 2 U1 6 U2 20 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAR 14 PY 2015 VL 142 IS 10 AR 101901 DI 10.1063/1.4906046 PG 7 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CD3KT UT WOS:000350978000002 PM 25770490 ER PT J AU Burmistrova, PV Zakharov, DN Favaloro, T Mohammed, A Stach, EA Shakouri, A Sands, TD AF Burmistrova, Polina V. Zakharov, Dmitri N. Favaloro, Tela Mohammed, Amr Stach, Eric A. Shakouri, Ali Sands, Timothy D. TI Effect of deposition pressure on the microstructure and thermoelectric properties of epitaxial ScN(001) thin films sputtered onto MgO(001) substrates SO JOURNAL OF MATERIALS RESEARCH LA English DT Article ID SCANDIUM NITRIDE FILMS; EVOLUTION; GROWTH; SCN; SILICON; VIEW AB Four epitaxial ScN(001) thin films were successfully deposited on MgO(001) substrates by dc reactive magnetron sputtering at 2, 5, 10, and 20 mTorr in an Ar/N-2 ambient atmosphere at 650 degrees C. The microstructure of the resultant films was analyzed by x-ray diffraction, scanning electron microscopy, and transmission electron microscopy. Electrical resistivity, electron mobility and concentration were measured using the room temperature Hall technique, and temperature dependent in-plain measurements of the thermoelectric properties of the ScN thin films were performed. The surface morphology and film crystallinity significantly degrade with increasing deposition pressure. The ScN thin film deposited at 20 mTorr exhibits the presence of <221> oriented secondary grains resulting in decreased electric properties and a low thermoelectric power factor of 0.5 W/mK(2) at 800 K. The ScN thin films grown at 5 and 10 mTorr are single crystalline, yielding the power factor of approximately 2.5 W/mK(2) at 800 K. The deposition performed at 2 mTorr produces the highest quality ScN thin film with the electron mobility of 98 cm(2) V-1 s(-1) and the power factor of 3.3 W/mK(2) at 800 K. C1 [Burmistrova, Polina V.; Mohammed, Amr; Shakouri, Ali; Sands, Timothy D.] Purdue Univ, Sch Elect & Comp Engn, W Lafayette, IN 47907 USA. [Burmistrova, Polina V.; Zakharov, Dmitri N.; Mohammed, Amr; Shakouri, Ali; Sands, Timothy D.] Purdue Univ, Birck Nanotechnol Ctr, W Lafayette, IN 47907 USA. [Zakharov, Dmitri N.; Stach, Eric A.] Brookhaven Natl Lab, Upton, NY 11974 USA. [Favaloro, Tela; Shakouri, Ali] Univ Calif Santa Cruz, Sch Engn, Santa Cruz, CA 95064 USA. [Sands, Timothy D.] Purdue Univ, Sch Mat Engn, W Lafayette, IN 47907 USA. RP Burmistrova, PV (reprint author), Purdue Univ, Sch Elect & Comp Engn, W Lafayette, IN 47907 USA. EM polina.burmistrova@stonybrook.edu RI Sands, Timothy/D-2133-2009; Stach, Eric/D-8545-2011; Zakharov, Dmitri/F-4493-2014 OI Sands, Timothy/0000-0001-9718-6515; Stach, Eric/0000-0002-3366-2153; FU DARPA/Army Research Office [W911NF0810347]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX This work was funded by DARPA/Army Research Office Contract No. W911NF0810347. Research carried out in part at the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. NR 37 TC 3 Z9 3 U1 5 U2 20 PU CAMBRIDGE UNIV PRESS PI NEW YORK PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA SN 0884-2914 EI 2044-5326 J9 J MATER RES JI J. Mater. Res. PD MAR 14 PY 2015 VL 30 IS 5 BP 626 EP 634 DI 10.1557/jmr.2015.30 PG 9 WC Materials Science, Multidisciplinary SC Materials Science GA CD9UO UT WOS:000351444200004 ER PT J AU Coffman, E Richmond-Bryant, J AF Coffman, Evan Richmond-Bryant, Jennifer TI Multiple biomarker models for improved risk estimation of specific cardiovascular diseases related to metabolic syndrome: a cross-sectional study SO POPULATION HEALTH METRICS LA English DT Article DE Cardiovascular disease; Biomarkers; Metabolic syndrome; Joint associations; NHANES ID C-REACTIVE PROTEIN; CORONARY-HEART-DISEASE; MYOCARDIAL-INFARCTION; FOLLOW-UP; STROKE; TRIGLYCERIDES; EPIDEMIOLOGY; ASSOCIATION; CHOLESTEROL; PREDICTION AB Background: Metabolic syndrome (MetS) is the co-occurrence of several conditions that increase risk of chronic disease and mortality. Multivariate models for calculating risk of MetS-related diseases based on combinations of biomarkers are promising for future risk estimation if based on large population samples. Given biomarkers' nonspecificity and commonality in predicting diseases, we hypothesized that unique combinations of the same clinical diagnostic criteria can be used in different multivariate models to develop more accurate individual and cumulative risk estimates for specific MetS-related diseases. Methods: We utilized adult biomarker and cardiovascular disease (CVD) data from the National Health and Nutrition Examination Survey as part of a cross-sectional analysis. Serum C-reactive protein (CRP), glycohemoglobin, triglycerides, high-density lipoprotein cholesterol, low-density lipoprotein cholesterol, total cholesterol, fasting glucose, and apolipoprotein-B were modeled. CVDs included congestive heart failure, coronary heart disease, angina, myocardial infarction, and stroke. Decile analysis for disease prevalence in each biomarker group and multivariate logistic regression for estimation of odds ratios were employed to measure the joint association between multiple biomarkers and CVD diagnoses. Results: Of the biomarkers considered, glycohemoglobin, triglycerides, and CRP were consistently associated with the CVD outcomes of interest in decile analysis and were selected for the final models. Associations were overestimated when using single-marker models in comparison with full models; individual odds ratios decreased an average of 16.4% from the single-biomarker models to the joint association models for CRP, 6.6% for triglycerides, and 1.4% for glycohemoglobin. However, joint associations were stronger than any single-marker estimate. Additionally, reduced models produced unique combinations of biomarkers for specific CVD outcomes. Conclusion: The reduced joint association modeling results suggest that unique combinations of biomarkers with their related measure of association can be used to produce more accurate cumulative risk estimates for each CVD. Additionally, our results indicate that the use of multiple biomarkers in a single multivariate model may provide increased accuracy of individual biomarker association estimates by controlling for statistical artifacts and spurious relationships due to co-biomarker confounding. C1 [Coffman, Evan] US EPA, Natl Ctr Environm Assessment, Oak Ridge Inst Sci & Educ, Environm Media Assessment Grp, Res Triangle Pk, NC 27711 USA. [Richmond-Bryant, Jennifer] US EPA, Environm Media Assessment Grp, Natl Ctr Environm Assessment, Res Triangle Pk, NC 27711 USA. RP Coffman, E (reprint author), US EPA, Natl Ctr Environm Assessment, Oak Ridge Inst Sci & Educ, Environm Media Assessment Grp, Mail Drop B243-01, Res Triangle Pk, NC 27711 USA. EM coffman.evan@epa.gov NR 36 TC 6 Z9 7 U1 0 U2 5 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1478-7954 J9 POPUL HEALTH METR JI Popul. Health Metr. PD MAR 14 PY 2015 VL 13 AR 7 DI 10.1186/s12963-015-0041-5 PG 15 WC Public, Environmental & Occupational Health SC Public, Environmental & Occupational Health GA CD7LZ UT WOS:000351273200001 PM 25788869 ER PT J AU Gaillard, MK AF Gaillard, Mary K. TI Perspective on the weakly coupled heterotic string SO MODERN PHYSICS LETTERS A LA English DT Review ID EFFECTIVE LAGRANGIAN ANALYSIS; DEPENDENT GAUGE COUPLINGS; EFFECTIVE FIELD-THEORIES; DYNAMICAL SUPERSYMMETRY BREAKING; MODULAR INVARIANT SUPERGRAVITY; SIGMA-MODEL ANOMALIES; SUPERSTRING MODELS; TARGET-SPACE; YANG-MILLS; COSMOLOGICAL PROBLEMS AB Since the first "string revolution" of 1984, the weakly coupled E-8 circle times E-8 heterotic string theory has been a promising candidate for the underlying theory of the Standard Model. The particle spectrum and the issue of dilaton stabilization are reviewed. Specific models for hidden sector condensation and supersymmetry breaking are described and their phenomenological and cosmological implications are discussed. The importance of T-duality is emphasized. Theoretical challenges to finding a satisfactory vacuum, as well as constraints from LHC data are addressed. C1 [Gaillard, Mary K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Phys, Berkeley, CA 94720 USA. [Gaillard, Mary K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Theoret Phys Grp, Berkeley, CA 94720 USA. RP Gaillard, MK (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Phys, 50A-5101, Berkeley, CA 94720 USA. EM mkgaillard@lbl.gov FU Office of Energy Research, Office of High Energy and Nuclear Physics, Division of High Energy Physics of the U.S. Department of Energy [DE-AC03-76SF00098]; National Science Foundation [PHY-0098840] FX I wish to thank my many collaborators, especially Pierre Binetruy, Joel Giedt, Brent Nelson, Tom Taylor and Yi-Yen Wu, from whom I have learned a lot. This work was supported in part by the Director, Office of Energy Research, Office of High Energy and Nuclear Physics, Division of High Energy Physics of the U.S. Department of Energy under Contract DE-AC03-76SF00098 and in part by the National Science Foundation under grant PHY-0098840. NR 108 TC 0 Z9 0 U1 0 U2 2 PU WORLD SCIENTIFIC PUBL CO PTE LTD PI SINGAPORE PA 5 TOH TUCK LINK, SINGAPORE 596224, SINGAPORE SN 0217-7323 EI 1793-6632 J9 MOD PHYS LETT A JI Mod. Phys. Lett. A PD MAR 14 PY 2015 VL 30 IS 8 AR 1530005 DI 10.1142/S0217732315300050 PG 22 WC Physics, Nuclear; Physics, Particles & Fields; Physics, Mathematical SC Physics GA CC7SZ UT WOS:000350570000001 ER PT J AU Lequieu, JP Hinckley, DM de Pablo, JJ AF Lequieu, Joshua P. Hinckley, Daniel M. de Pablo, Juan J. TI A molecular view of DNA-conjugated nanoparticle association energies SO SOFT MATTER LA English DT Article ID CRYSTALLIZATION; SUPERLATTICES; HYBRIDIZATION AB Nanoparticles functionalized with short sequences of DNA represent a promising platform for customizable self assembly. Though much recent research has focused on the phase behavior and assembly of these structures, little has been done to precisely characterize the pairwise interaction between particles. Here we present a detailed calculation of the association between DNA-nanoparticle conjugates using 3SPN. 2, a coarse-grained model of DNA that accounts for molecular structure and base-pairing. We compare our results to those obtained experimentally using mm sized particles and analyze the free energy surfaces that characterize interparticle hybridization. Next, we study the importance of three-body effects and their impact on particle association and melting. Lastly, we explore the observation by Park et al. [Nature, 451, 553 (2008)] that DNA-nanoparticle crystallization can be inhibited by the deletion of a single nucleotide. Using our model, we suggest that the role of this nucleotide is to disrupt frustration. C1 [Lequieu, Joshua P.; de Pablo, Juan J.] Univ Chicago, Inst Mol Engn, Chicago, IL 60637 USA. [Hinckley, Daniel M.] Univ Wisconsin, Dept Chem & Biol Engn, Madison, WI 53706 USA. [de Pablo, Juan J.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP de Pablo, JJ (reprint author), Univ Chicago, Inst Mol Engn, Chicago, IL 60637 USA. EM depablo@uchicago.edu FU NIST through the Center for Hierarchical Materials Assembly (CHiMaD); NSF-supported Nansocale Science and Engineering Center (NSEC); National Science Foundation [DGE-1256259] FX The authors thank Dr Gordon S. Freeman and Dr Jonathan K. Whitmer for helpful discussions. We further acknowledge computational resources provided by the Midway computing cluster at the University of Chicago. J.P.L. gratefully acknowledges support of this research by NIST through the Center for Hierarchical Materials Assembly (CHiMaD). The original DNA models used for the calculations reported here were developed with support from the NSF-supported Nansocale Science and Engineering Center (NSEC). The University of Wisconsin-Madison Center for High Throughput Computing is gratefully acknowledged for providing computational resources and computer expertise. D.M.H. was funded by a Graduate Research Fellowship from the National Science Foundation (grant no. DGE-1256259). NR 32 TC 4 Z9 4 U1 2 U2 19 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1744-683X EI 1744-6848 J9 SOFT MATTER JI Soft Matter PD MAR 14 PY 2015 VL 11 IS 10 BP 1919 EP 1929 DI 10.1039/c4sm02573c PG 11 WC Chemistry, Physical; Materials Science, Multidisciplinary; Physics, Multidisciplinary; Polymer Science SC Chemistry; Materials Science; Physics; Polymer Science GA CC9HM UT WOS:000350679300007 PM 25611690 ER PT J AU Aad, G Abbott, B Abdallah, J Khalek, SA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Agatonovic-Jovin, T Aguilar-Saavedra, JA Agustoni, M Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TP Akimoto, G Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Allbrooke, BMM Allison, LJ Allport, PP Almond, J Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Anduaga, XS Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonaki, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Apolle, R Arabidze, G Aracena, I Arai, Y Araque, JP Arce, ATH Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Arnaez, O Arnal, V Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Asai, S Asbah, N Ashkenazi, A Asman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Auerbach, B Augsten, K Aurousseau, M Avolio, G Azuelos, G Azuma, Y Baak, MA Bacci, C Bachacou, H Bachas, K Backes, M Backhaus, M Mayes, JB Badescu, E Bagiacchi, P Bagnaia, P Bai, Y Bain, T Baines, JT Baker, OK Baker, S Balek, P Balli, F Banas, E Banerjee, S Bannoura, AAE Bansal, V Bansil, HS Barak, L Baranov, SP Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, P Bartsch, V Bassalat, A Basye, A Bates, RL Batkova, L Batley, JR Battaglia, M Battistin, M Bauer, F Bawa, HS Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, S Beckingham, M Becot, C Beddall, AJ Beddall, A Bedikian, S Bednyakov, VA Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, K Belanger-Champagne, C Bell, PJ Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belotskiy, K Beltramello, O Benary, O Benchekrouna, D Bendtza, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Benslama, K Bentvelsen, S Berge, D Kuutmann, EB Berger, N Berghaus, F Berglund, E Beringer, J Bernard, C Bernat, P Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertoli, G Bertolucci, F Bertsche, D Besana, MI Besjes, GJ Bylund, OB Bessner, M Besson, N Betancourt, C Bethke, S Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Bieniek, SP Bierwagen, K Biesiada, J Bigliettia, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Black, CW Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blazek, T Bloch, I Blocker, C Blum, W Blumenschein, U Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Bock, C Boddy, CR Boehler, M Boek, J Boek, TT Bogaerts, JA Bogdanchikov, AG Bogouch, A Bohm, C Bohm, J Boisvert, V Bold, T Boldea, V Boldyrev, AS Bomben, M Bona, M Boonekamp, M Borisov, A Borissov, G Borri, M Borroni, S Bortfeldt, J Bortolotto, V Bos, K Boscherini, D Bosman, M Boterenbrood, H Boudreau, J Bouffard, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boutouild, S Boveia, A Boyd, J Boyko, IR Bozovic-Jelisavcic, I Bracinik, J Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Brazzale, SF Brelier, B Brendlinger, K Brennan, AJ Brenner, R Bressler, S Bristow, K Bristow, TM Britton, D Brochu, FM Brock, I Brock, R Bromberg, C Bronner, J Brooijmans, G Brooks, T Brooks, WK Brosamer, J Brost, E Brown, G Brown, J de Renstrom, PAB Bruncko, D Bruneliere, R Brunet, S Bruni, A Bruni, G Bruschi, M Bryngemark, L Buanes, T Buat, Q Bucci, F Buchholz, P Buckingham, RM Buckley, AG Buda, SI Budagov, IA Buehrer, F Bugge, L Bugge, MK Bulekov, O Bundock, AC Burckhart, H Burdin, S Burghgrave, B Burke, S Burmeister, I Busato, E Buescher, D Buescher, V Bussey, P Buszello, CP Butler, B Butler, JM Butt, AI Buttar, CM Butterworth, JM Butti, P Buttinger, W Buzatu, A Byszewski, M Urban, SC Caforio, D Cakir, O Calafiura, P Calandri, A Calderini, G Calfayan, P Calkins, R Caloba, LP Calvet, D Calvet, S Toro, RC Camarda, S Cameron, D Caminada, LM Armadans, RC Campana, S Campanelli, M Campoverde, A Canale, V Canepa, A Bret, MC Cantero, J Cantrill, R Cao, T Garrido, MDMC Caprini, I Caprini, M Capua, M Caputo, R Cardarelli, R Carli, T Carlino, G Carminati, L Caron, S Carquin, E Carrillo-Montoya, GD Carter, JR Carvalho, J Casadei, D Casado, MP Casolino, M Castaneda-Miranda, E Castelli, A Gimenez, VC Castro, NF Catastini, P Catinaccio, A Catmore, JR Cattai, A Cattani, G Caughron, S Cavaliere, V Cavalli, D Cavalli-Sforza, M Cavasinnia, V Ceradini, F Cerio, B Cerny, K Cerqueira, AS Cerri, A Cerrito, L Cerutti, F Cerv, M Cervelli, A Cetin, SA Chafaq, A Chakraborty, D Chalupkova, I Chan, K Chang, P Chapleau, B Chapman, JD Charfeddine, D Charlton, DG Chau, CC Barajas, CAC Cheatham, S Chegwidden, A Chekanov, S Chekulaev, SV Chelkov, GA Chelstowska, MA Chen, C Chen, H Chen, K Chen, L Chen, S Chen, X Chen, Y Cheng, HC Cheng, Y Cheplakov, A El Mourslie, RC Chernyatin, V Cheu, E Chevalier, L Chiarella, V Chiefari, G Childers, JT Chilingarov, A Chiodini, G Chisholm, AS Chislett, RT Chitan, A Chizhov, MV Chouridou, S Chow, BKB Chromek-Burckhart, D Chu, ML Chudoba, J Chwastowski, JJ Chytka, L Ciapetti, G Ciftci, AK Ciftci, R Cinca, D Cindro, V Ciocio, A Cirkovic, P Citron, ZH Citterio, M Ciubancan, M Clark, A Clark, PJ Clarke, RN Cleland, W Clemens, JC Clement, C Coadou, Y Cobal, M Coccaro, A Cochran, J Coffey, L Cogan, JG Coggeshall, J Cole, B Cole, S Colijn, AP Collot, J Colombo, T Colon, G Compostella, G Muino, PC Coniavitis, E Conidi, MC Connell, SH Connelly, IA Consonni, SM Consorti, V Constantinescu, S Conta, C Conti, G Conventi, F Cooke, M Cooper, BD Cooper-Sarkar, AM Cooper-Smith, NJ Copic, K Cornelissen, T Corradi, M Corriveau, F Corso-Radu, A Cortes-Gonzalez, A Cortiana, G Costa, G Costa, MJ Costanzo, D Cote, D Cottin, G Cowan, G Cox, BE Cranmer, K Cree, G Crepe-Renaudin, S Crescioli, F Cribbs, WA Ortuzar, MC Cristinziani, M Croft, V Crosetti, G Cuciuc, CM Donszelmann, TC Cummings, J Curatolo, M Cuthbert, C Czirr, H Czodrowski, P Czyczula, Z D'Auria, S D'Onofrio, M De Sousa, MJDS Da Via, C Dabrowski, W Dafinca, A Dai, T Dale, O Dallaire, 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CA ATLAS Collaboration TI Performance of the ATLAS muon trigger in pp collisions at root s=8 TeV SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID BOSON; LHC AB The performance of the ATLAS muon trigger system is evaluated with proton-proton collision data collected in 2012 at the Large Hadron Collider at a centre-of-mass energy of 8TeV. It is primarily evaluated using events containing a pair of muons from the decay of Z bosons. The efficiency of the single-muon trigger is measured for muons with transverse momentum 25 < pT < 100 GeV, with a statistical uncertainty of less than 0.01% and a systematic uncertainty of 0.6%. The pT range for efficiency determination is extended by using muons from decays of J/Psi mesons, W bosons, and top quarks. The muon trigger shows highly uniform and stable performance. The performance is compared to the prediction of a detailed simulation. C1 [Jackson, P.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. 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A.; Hu, X.; Klimentov, A.; Kravchenko, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Metcalfe, J.; Mountricha, E.; Nevski, P.; Okawa, H.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Perepelitsa, D. V.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Schovancova, J.; Snyder, S.; Steinberg, P.; Takai, H.; Triplett, N.; Undrus, A.; Wenaus, T.; Ye, S.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Badescu, E.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Cuciuc, C. -M.; Dita, P.; Dita, S.; Ducua, O. A.; Jinaru, A.; Maurer, J.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorachea, A.; Tudorachea, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Gonzalez Silva, M. L.; Otero Y Garzon, G.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Buttinger, W.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Frost, J. A.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Moeller, V.; Mueller, T.; Parker, M. A.; Robinson, D.; Sandoval, T.; Thomson, M.; Ward, C. P.; Williams, S.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Leight, W. A.; Marchand, J. F.; McCarthy, T. G.; Oakham, F. G.; Pasztor, G.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Abreu, R.; Aleksa, M.; Andari, N.; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Battistin, M.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Dell'Acqua, A.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dopke, J.; Dudarev, A.; Duehrssen, M.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Perez, S. Fernandez; Franchino, S.; Francis, D.; Froidevaux, D.; Garonne, V.; Gianotti, F.; Gillberg, D.; Glatzer, J.; Godlewski, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hauschild, M.; Hawkings, R. J.; Heller, M.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Hubacek, Z.; Huhtinen, M.; Jaekel, M. R.; Jakobsen, S.; Jansen, H.; Jungst, R. M.; Kaneda, M.; Klioutchnikova, T.; Krasznahorkay, A.; Lantzsch, K.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Martin, B.; Marzin, A.; Messina, A.; Meyer, J.; Milic, A.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Negri, G.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Ohm, C. C.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Rodrigues, L.; Roe, S.; Ruiz-Martinez, A.; Salzburger, A.; Savu, D. O.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; Van der Ster, D.; Van Eldik, N.; Van Woerden, M. C.; Vandelli, W.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Boveia, A.; Cheng, Y.; Facini, G.; Fiascaris, M.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Li, H. L.; Meehan, S.; Melachrinos, C.; Merritt, F. S.; Meyer, C.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Shochet, M. J.; Tompkins, L.; Vukotic, I.; Webster, J. S.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carquin, E.; Diaz, M. A.; Vogela, M.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; Whiteb, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fanga, Y.; Jin, S.; Lu, F.; Ouyang, Q.; Ren, H.; Shan, L. Y.; Sun, X.; Wanga, J.; Xua, D.; Yaoa, L.; Zhua, H.; Zhuanga, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guan, L.; Han, L.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, K.; Liu, M.; Liu, Y.; Peng, H.; Song, H. Y.; Xub, L.; Zhaob, Z.; Zhub, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.] Nanjing Univ, Dept Phys, Nanjing 210008, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Ma, L. L.; Zhangd, X.; Zhud, C. G.] Shandong Univ, Sch Phys, Jinan 250100, Shandong, Peoples R China. [Li, L.; Li, Y.; Yange, H.] Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200030, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Clermont Univ, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Photochim Mol & Macromol Lab, CNRS, IN2P3, F-63177 Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Chen, Y.; Cole, B.; Guo, J.; Hu, D.; Hughes, E. W.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Reale, V. Perez; Scherzer, M. I.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Wulf, E.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Heisterkamp, S.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Mehlhase, S.; Monk, J.; Petersen, T. C.; Pingel, A.; Simonyan, M.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, DK-2100 Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Nazl Frascati Lab, Grp Coll Cosenza, I-00044 Frascati, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemlaa, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Palka, M.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hoffman, J.; Kama, S.; Keil, M.; Randle-Conde, A. S.; Sekula, S. J.; Stroynowski, R.; Wang, H.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Lou, X.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Camarda, S.; Dassoulas, J. A.; Deterre, C.; Dietrich, J.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Belenguer, M. Jimenez; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Medinnis, M.; Moenig, K.; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Hamburg, Germany. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Camarda, S.; Dassoulas, J. A.; Deterre, C.; Dietrich, J.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Belenguer, M. Jimenez; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Medinnis, M.; Moenig, K.; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Wittig, T.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Kobel, M.; Leonhardt, K.; Mader, W. F.; Morgenstern, M.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Pollard, C. S.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Debenedetti, C.; Edwards, N. C.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Di Simone, A.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Prokofiev, K.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Buescher, D.; Consorti, V.; Fehling-Kaschek, M.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Madar, R.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Rave, T. C.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; Von Radziewski, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Alexandre, G.; Ancu, L. S.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Bucci, F.; Toro, R. Camacho; Clark, A.; Delitzsch, C. M.; della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; LaRosa, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Nektarijevic, S.; Nikolics, K.; Picazio, A.; Pohl, M.; Rosbach, K.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] INFN Sez Genova, Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadzea, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Bates, R. L.; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; Saxon, D. H.; Smith, K. M.; St Denis, R. D.; Stewart, G. A.; Thompson, A. S.; Wright, M.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bierwagen, K.; Bindi, M.; Blumenschein, U.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Hensel, C.; Kawamura, G.; Kehoe, R.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Stolte, P.; Schroeder, T. Vazquez; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Butler, B.; Catastini, P.; Conti, G.; Franklin, M.; Huth, J.; Ippolito, V.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Yen, A. L.; Della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Brandt, O.; Davygora, Y.; Dietzsch, T. A.; Dunford, M.; Hanke, P.; Hofmann, J. I.; Jongmanns, J.; Khomich, A.; Kluge, E. -E.; Laier, H.; Lang, V. S.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wesselsa, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Franz, S.; Jussel, P.; Kneringer, E.; Lukas, W.; Nagai, K.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Cinca, D.; Gandrajula, R. P.; Ikegami, Y.; Mallik, U.; Mandrysch, R.; Morange, N.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Kazarinov, M. Y.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Mitsui, S.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Inamaru, Y.; Kishimoto, T.; Kitamura, T.; Kurashige, H.; Kurumida, R.; Matsushita, T.; Ochi, A.; Shimizu, S.; Takeda, H.; Tani, K.; Watanabe, I.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Verzini, M. J. Alconada; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, RA-1900 La Plata, Buenos Aires, Argentina. [Verzini, M. J. Alconada; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Allison, L. J.; Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Venturaa, A.] INFN Sez Lecce, Lecce, Italy. [Gorini, E.; Orlando, N.; Spagnolo, S.; Venturaa, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Readioff, N. P.; Schnellbach, Y. J.; Sellers, G.; Vossebeld, J. H.; Waller, P.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bona, M.; Bret, M. Cano; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Rizvi, E.; Salamanna, G.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Boisvert, V.; Brooks, T.; Cantrill, R.; Connelly, I. A.; Cooper-Smith, N. J.; Cowan, G.; Duguid, L.; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Baker, S.; Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Cooper, B. D.; Davison, A. R.; Davison, P.; Falla, R. J.; Gregersen, K.; Gutschow, C.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Korn, A.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, M. I.; Pilkington, A. D.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Bernius, C.; Greenwood, Z. D.; Jana, D. K.; Sawyer, L.; Sircar, A.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; LeDortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Rose, M.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; LeDortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Rose, M.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; LeDortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Rose, M.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS IN2P3, Paris, France. [Akesson, T. P.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Meirose, B.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fysiska Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Blum, W.; Buescher, V.; Caputo, R.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Goeringer, C.; Heck, T.; Hohlfeld, M.; Hsu, P. J.; Huelsing, T. A.; Ji, W.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lin, T. H.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Meyer, C.; Moreno, D.; Moritz, S.; Mueller, T.; Poettgen, R.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, D-55122 Mainz, Germany. [Almond, J.; Borri, M.; Brown, G.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Peters, R. F. Y.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Robinson, J. E. M.; Schwanenberger, C.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Bertella, C.; Clemens, J. C.; Coadou, Y.; Diglio, S.; Djama, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; LeGuirriec, E.; Li, B.; Limosani, A.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Bertella, C.; Clemens, J. C.; Coadou, Y.; Diglio, S.; Djama, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; LeGuirriec, E.; Li, B.; Limosani, A.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] CNRS IN2P3, Marseille, France. [Bellomo, M.; Brau, B.; Colon, G.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Mantifel, R.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Jennens, D.; Kubota, T.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Shao, Q. T.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Urquijo, P.; Volpi, M.] Univ Melbourne, Sch Phys, Parkville, Vic 3052, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Dubbert, J.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Harper, D.; Levin, D.; Liu, L.; Long, J. D.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Panikashvili, N.; Qian, J.; Searcy, J.; Thun, R. P.; Wilson, A.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Alvarez Gonzalez, B.; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Koll, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Citterio, M.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Meloni, F.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turraa, R.; Pereza, M. Villaplana] INFN Sez Milano, Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Meloni, F.; Perini, L.; Pizio, C.; Ragusa, F.; Simoniello, R.; Turraa, R.; Pereza, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Acad Sci, PN Lebedev Inst Phys, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.; Vorobev, K.] Moscow Engn & Phys Inst MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Becker, S.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Ebke, J.; Elmsheuser, J.; Heller, C.; Hertenberger, R.; Legger, F.; Lorenz, J.; Mann, A.; Meineck, C.; Mitrevski, J.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Schieck, J.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Will, J. Z.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Manfredini, A.; Menke, S.; Moser, H. G.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Pahl, C.; Pospelov, G. E.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Stern, S.; Stonjek, S.; Terzo, S.; Von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci & Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Chiefari, G.; Conventi, F.; De Asmundisa, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Giordano, R.; Iengo, P.; Izzoa, V.; Merola, L.; Patricelli, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] INFN Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Chiefari, G.; Di Donato, C.; Giordano, R.; Merola, L.; Patricelli, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Croft, V.; Dao, V.; De Groot, N.; Filthaut, F.; Galea, C.; Klok, P. F.; Koenig, A. C.; Salvucci, A.] Radboud Univ Nijmegen, Nikhef, Inst Math Astrophys & Particle Phys, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Butti, P.; Castelli, A.; Colijn, A. P.; Jong, P. de; De Nooij, L.; Deigaard, I.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Oussoren, K. P.; Pani, P.; Salek, D.; Valencic, N.; Van der Deijl, P. C.; Van der Geer, R.; Van der Graaf, H.; Van der Leeuw, R.; Van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Butti, P.; Castelli, A.; Colijn, A. P.; Jong, P. de; De Nooij, L.; Deigaard, I.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Oussoren, K. P.; Pani, P.; Salek, D.; Valencic, N.; Van der Deijl, P. C.; Van der Geer, R.; Van der Graaf, H.; Van der Leeuw, R.; Van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Univ Amsterdam, Amsterdam, Netherlands. [Burghgrave, B.; Calkins, R.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL USA. [Anisenkov, A. V.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Skovpen, K. Yu.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Korol, A. A.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, New York, NY 10003 USA. [Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Bertsche, D.; Gutierrez, P.; Hasib, A.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Bousson, N.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] CNRS IN2P3, Orsay, France. [Endo, M.; Hanagaki, K.; Lee, J. S. H.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Brau, J. E.; Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Gjelsten, B. K.; Gramstad, E.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Read, A. L.; Rohne, O.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Apolle, R.; Barr, A. J.; Behr, K.; Boddy, C. R.; Buckingham, R. M.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; King, R. S. B.; Kogan, L. A.; Lewis, A.; Livermore, S. S. A.; Nickerson, R. B.; Pachal, K.; Pinder, A.; Ryder, N. C.; Sawyer, C.; Short, D.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesia, V.] INFN Sez Pavia, Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Ospanov, R.; Saxon, J.; Schaefer, D.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Vanguri, R.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Roda, C.; Scuri, F.; Volpia, G.; Whitea, S.] INFN Sez Pisa, Pisa, Italy. [Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Roda, C.; Scuri, F.; Volpia, G.; Whitea, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Kittelmann, T.; Mueller, J.; Prieur, D.; Sapp, K.; Su, J.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Dos Santos, S. P. Amor; Amorim, A.; Anjos, N.; Araque, J. P.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Wemans, A. Do Valle; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Miguens, J. Machado; Maio, A.; Maneira, J.; Marquesa, C. N.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Velosoa, F.; Woltersa, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Dos Santos, S. P. Amor; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Velosoa, F.; Woltersa, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. [Wemans, A. Do Valle] Univ Nova Lisboa, Dep Fis, Caparica, Portugal. [Wemans, A. Do Valle] Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, Caparica, Portugal. [Bohm, J.; Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Gallus, P.; Gunther, J.; Jakubek, J.; Kohout, Z.; Kral, V.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Leitner, R.; Pleskot, V.; Reznicek, P.; Rybar, M.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] State Res Ctr Inst High Energy Phys, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Benslama, K.] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Dionisi, C.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Sidoti, A.; Camillocci, E. Solfaroli; Vanadiaa, M.; Varia, R.; Venezianoa, S.; Zanelloa, L.] INFN Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; Di Domenico, A.; Dionisi, C.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Monzani, S.; Camillocci, E. Solfaroli; Vanadiaa, M.; Zanelloa, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Iuppa, R.; Liberti, B.; Mazzaferro, L.; Paolozzi, L.; Salamon, A.; Santonico, R.] INFN Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Iuppa, R.; Mazzaferro, L.; Paolozzi, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Bigliettia, M.; Bortolotto, V.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Stanescu, C.; Trovatelli, M.] INFN Sez Roma Tre, Rome, Italy. [Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekrouna, D.; Chafaq, A.; Giordani, M. P.; Gouighri, M.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA Marrakech, Fac Sci Semlalia, Marrakech, Morocco. [Boutouild, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Boutouild, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Mourslie, R. Cherkaoui; Fassi, F.; Haddad, N.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Grabas, H. M. X.; Guyot, C.; Hanna, R.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mal, P.; Mansoulie, B.; Martinez, H.; Meric, N.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.; Tsionou, D.; Vranjes, N.; Xiao, M.] CEA Saclay Commissariat Energie Atom & Energie Al, DSM IRFU, Inst Rech Lois Fondament Univers, Gif Sur Yvette, France. [Battaglia, M.; Grillo, A. A.; Kuhl, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Beckingham, M.; Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; De Bruin, P. H. Sales; Verducci, M.; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Paredes, B. Lopez; Miyagawa, P. S.; Paganis, E.; Suruliz, K.; Tovey, D. R.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Dawe, E.; Godfrey, J.; O'Neil, D. C.; Petteni, M.; Stelzer, B.; Tanasijczuk, A. J.; Torres, H.; Trottier-McDonald, M.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Mayes, J. Backus; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Kagan, M.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nelson, T. K.; Piacquadio, G.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Strauss, E.; Su, D.; Swiatlowski, M.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Batkova, L.; Blazek, T.; Federic, P.; Plazak, L.; Stavina, P.; Sykora, I.; Tokar, S.; Zenisa, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Connell, S. H.; Yacoobb, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Carrillo-Montoya, G. D.; Chen, X.; Mellado Garcia, B. R.; Ruan, X.; Vickeyc, T.; Boeriuc, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtza, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Silverstein, S. B.; Sjoelin, J.; Strandberg, S.; Tylmada, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtza, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Gellerstedt, K.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Sjoelin, J.; Strandberg, S.; Tylmada, M.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys, Stony Brook, NY 11794 USA. [Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Astron, Stony Brook, NY 11794 USA. [Bartsch, V.; Cerri, A.; Barajas, C. A. Chavez; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Chu, M. L.; Hou, S.; Jamin, D. O.; Lee, C. A.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; LoSterzo, F.; Mazini, R.; Ren, Z. L.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, C.; Wang, S. M.; Weng, Z.; Zhang, L.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Guttman, N.; Munwes, Y.; Oren, Y.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kordas, K.; Kouskoura, V.; Leisos, A.; Nomidis, I.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kanno, T.; Kobayashi, D.; Kuze, M.; Nagai, R.; Nobe, T.; Pettersson, N. E.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Brelier, B.; Chau, C. C.; Ilic, N.; Keung, J.; Krieger, P.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Schramm, S.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Chekulaev, S. V.; Fortin, D.; Koutsman, A.; Oram, C. J.; Codina, E. Perez; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Bustos, A. C. Florez; Ramos, J. A. Manjarres; Palacino, G.; Qureshi, A.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Farrell, S.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Rao, K.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Pinamonti, M.; Quayle, W. B.; Shaw, K.; Soualah, R.] INFN Grp Coll Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; De Sanctis, U.; Pinamonti, M.; Quayle, W. B.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Alhroob, M.; Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Coggeshall, J.; Errede, D.; Errede, S.; Lie, K.; Liss, T. M.; Neubauer, M. S.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Brenner, R.; Buszello, C. P.; Coniavitis, E.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.; Valero, A.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Urban, S. Cabrera; Castillo Gimenez, V.; Costa, M. J.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Urban, S. Cabrera; Castillo Gimenez, V.; Costa, M. J.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Urban, S. Cabrera; Castillo Gimenez, V.; Costa, M. J.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Urban, S. Cabrera; Castillo Gimenez, V.; Costa, M. J.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Urban, S. Cabrera; Castillo Gimenez, V.; Costa, M. J.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] CSIC, Valencia, Spain. [Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Loh, C. W.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Bansal, V.; Berghaus, F.; Bernlochner, F. U.; David, C.; Fincke-Keeler, M.; Hamano, K.; Hill, E.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Marino, C. P.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.; Venturi, M.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Farrington, S. M.; Harrison, P. F.; Janus, M.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Kimura, N.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Barak, L.; Bressler, S.; Citron, Z. H.; Duchovni, E.; Gabizon, O.; Gross, E.; Groth-Jensen, J.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Milstein, D.; Pitt, M.; Roth, I.; Schaarschmidt, J.; Smakhtin, V.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Castillo, L. R. Flores; Hard, A. S.; Ji, H.; Ju, X.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Redelbach, A.; Schreyer, M.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Bannoura, A. A. E.; Barisonzi, M.; Becker, K.; Beermann, T. A.; Boek, J.; Boek, T. T.; Braun, H. M.; Cornelissen, T.; Duda, D.; Ernis, G.; Fischer, J.; Fleischmann, S.; Flick, T.; Hamacher, K.; Harenberg, T.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Khoroshilov, A.; Kohlmann, S.; Lenzen, G.; Maetig, P.; Neumann, M.; Pataraia, S.; Sandhoff, M.; Sartisohn, G.; Wagner, W.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany. [Adelman, J.; Baker, O. K.; Bedikian, S.; Cummings, J.; Czyczula, Z.; Demers, S.; Erdmann, J.; Garberson, F.; Golling, T.; Guest, D.; Henrichs, A.; Ideal, E.; Lagouri, T.; Lee, L.; Leister, A. G.; Loginov, A.; Tipton, P.; Wall, R.; Walsh, B.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] IN2P3, Ctr Calcul, Villeurbanne, France. [Acharya, B. S.] Kings Coll London, Dept Phys, London WC2R 2LS, England. [Ahmadov, F.; Huseynov, N.; Javadov, N.] Azerbaijan Acad Sci, Inst Phys, Baku 370143, Azerbaijan. [Apolle, R.; Davies, E.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Azuelos, G.; Gingrich, D. M.; Oakham, F. G.; Savard, P.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Bawa, H. S.; Gao, Y. S.; Lowe, A. J.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Chelkov, G. A.] Tomsk State Univ, Tomsk 634050, Russia. [Chen, L.; Gao, J.] Aix Marseille Univ, CPPM, Marseille, France. [Chen, L.; Gao, J.] CNRS IN2P3, Marseille, France. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Corriveau, F.; McPherson, R. A.; Robertson, S. H.; Sobie, R.; Teuscher, R. J.] IPP, Toronto, ON, Canada. [Fedin, O. L.] St Petersburg State Polytech Univ, Dept Phys, St Petersburg, Russia. [Castillo, L. R. Flores] Chinese Univ Hong Kong, Hong Kong, Hong Kong, Peoples R China. [Gkialas, I.; Papageorgiou, K.] Univ Aegean, Dept Financial & Management Engn, Chios, Greece. [Greenwood, Z. D.; Sawyer, L.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Grinstein, S.; Rozas, A. Juste; Martinez, M.] ICREA, Barcelona, Spain. [Ilchenko, Y.; Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Jejelava, J.] Ilia State Univ, Inst Theoret Phys, Tbilisi, Rep of Georgia. [Jenni, P.] CERN, Geneva, Switzerland. [Kono, T.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo 112, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Korol, A. A.; Maximov, D. A.; Rezanova, O. L.; Talyshev, A. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Li, B.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Li, Y.] Univ Paris 11, LAL, Orsay, France. [Li, Y.] CNRS IN2P3, Orsay, France. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei 115, Taiwan. [Liu, K.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Liu, K.] Univ Paris Diderot, Paris, France. [Liu, K.] CNRS IN2P3, Paris, France. [Mal, P.] Natl Inst Sci Educ & Res, Sch Phys Sci, Bhubaneswar, Orissa, India. [Messina, A.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Nessi, M.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Shi, L.; Soh, D. A.; Weng, Z.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Tikhomirov, V. O.] Moscow Engn & Phys Inst MEPhI, Moscow, Russia. [Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Vickeyc, T.] Univ Oxford, Dept Phys, Oxford, England. [Wang, C.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Wildt, M. A.] Univ Hamburg, Inst Expt Phys, Hamburg, Germany. [Xub, L.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Yacoobb, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. [ATLAS Collaboration] CERN, CH-1211 Geneva 23, Switzerland. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France. RI SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Olshevskiy, Alexander/I-1580-2016; Snesarev, Andrey/H-5090-2013; Kantserov, Vadim/M-9761-2015; Solfaroli Camillocci, Elena/J-1596-2012; Ippolito, Valerio/L-1435-2016; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; KHODINOV, ALEKSANDR/D-6269-2015; Staroba, Pavel/G-8850-2014; De, Kaushik/N-1953-2013; Carvalho, Joao/M-4060-2013; Mashinistov, Ruslan/M-8356-2015; Buttar, Craig/D-3706-2011; Smirnova, Oxana/A-4401-2013; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Wemans, Andre/A-6738-2012; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; Perrino, Roberto/B-4633-2010; Goncalo, Ricardo/M-3153-2016; Gauzzi, Paolo/D-2615-2009; Mindur, Bartosz/A-2253-2017; Gutierrez, Phillip/C-1161-2011; Gerbaudo, Davide/J-4536-2012; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Peleganchuk, Sergey/J-6722-2014; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Garcia, Jose /H-6339-2015; Tassi, Enrico/K-3958-2015; Boyko, Igor/J-3659-2013; Ciubancan, Liviu Mihai/L-2412-2015; Zhukov, Konstantin/M-6027-2015; Shmeleva, Alevtina/M-6199-2015; Gavrilenko, Igor/M-8260-2015; Tikhomirov, Vladimir/M-6194-2015; Moraes, Arthur/F-6478-2010; Chekulaev, Sergey/O-1145-2015; Warburton, Andreas/N-8028-2013; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; Livan, Michele/D-7531-2012; Bosman, Martine/J-9917-2014; Petrucci, Fabrizio/G-8348-2012; Negrini, Matteo/C-8906-2014; Costa, Maria Jose/H-5962-2015; Cavalli-Sforza, Matteo/H-7102-2015; Mitsou, Vasiliki/D-1967-2009; Di Domenico, Antonio/G-6301-2011; Grancagnolo, Sergio/J-3957-2015; Doyle, Anthony/C-5889-2009; Brooks, William/C-8636-2013; spagnolo, stefania/A-6359-2012; Della Pietra, Massimo/J-5008-2012 OI SULIN, VLADIMIR/0000-0003-3943-2495; Vykydal, Zdenek/0000-0003-2329-0672; Olshevskiy, Alexander/0000-0002-8902-1793; Kantserov, Vadim/0000-0001-8255-416X; Solfaroli Camillocci, Elena/0000-0002-5347-7764; Ippolito, Valerio/0000-0001-5126-1620; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; KHODINOV, ALEKSANDR/0000-0003-3551-5808; De, Kaushik/0000-0002-5647-4489; Carvalho, Joao/0000-0002-3015-7821; Mashinistov, Ruslan/0000-0001-7925-4676; Smirnova, Oxana/0000-0003-2517-531X; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Wemans, Andre/0000-0002-9669-9500; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; Perrino, Roberto/0000-0002-5764-7337; Goncalo, Ricardo/0000-0002-3826-3442; Gauzzi, Paolo/0000-0003-4841-5822; Mindur, Bartosz/0000-0002-5511-2611; Gerbaudo, Davide/0000-0002-4463-0878; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Boyko, Igor/0000-0002-3355-4662; Ciubancan, Liviu Mihai/0000-0003-1837-2841; Tikhomirov, Vladimir/0000-0002-9634-0581; Moraes, Arthur/0000-0002-5157-5686; Warburton, Andreas/0000-0002-2298-7315; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; Livan, Michele/0000-0002-5877-0062; Bosman, Martine/0000-0002-7290-643X; Petrucci, Fabrizio/0000-0002-5278-2206; Negrini, Matteo/0000-0003-0101-6963; Mitsou, Vasiliki/0000-0002-1533-8886; Di Domenico, Antonio/0000-0001-8078-2759; Grancagnolo, Sergio/0000-0001-8490-8304; Doyle, Anthony/0000-0001-6322-6195; Brooks, William/0000-0001-6161-3570; spagnolo, stefania/0000-0001-7482-6348; Della Pietra, Massimo/0000-0003-4446-3368 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union; ERC, European Union; NSRF, European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; ISF, Israel; MINERVA, Israel; GIF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; NCN, Poland; GRICES, Portugal; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; ISF, MINERVA, GIF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 26 TC 1 Z9 1 U1 5 U2 44 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD MAR 13 PY 2015 VL 75 IS 3 AR 120 DI 10.1140/epjc/s10052-015-3325-9 PG 31 WC Physics, Particles & Fields SC Physics GA CJ7HW UT WOS:000355666500002 ER PT J AU Portnichenko, PY Cameron, AS Surmach, MA Deen, PP Paschen, S Prokofiev, A Mignot, JM Strydom, AM Telling, MTF Podlesnyak, A Inosov, DS AF Portnichenko, P. Y. Cameron, A. S. Surmach, M. A. Deen, P. P. Paschen, S. Prokofiev, A. Mignot, J. -M. Strydom, A. M. Telling, M. T. F. Podlesnyak, A. Inosov, D. S. TI Momentum-space structure of quasielastic spin fluctuations in Ce3Pd20Si6 SO PHYSICAL REVIEW B LA English DT Article ID CEB6; COMPOUND; DIFFRACTION; SCATTERING; SYSTEMS; CEAL3 AB Among heavy-fermion metals, Ce3Pd20Si6 is one of the heaviest-electron systems known to date. Here we used high-resolution neutron spectroscopy to observe low-energy magnetic scattering from a single crystal of this compound in the paramagnetic state. We investigated its temperature dependence and distribution in momentum space, which was not accessible in earlier measurements on polycrystalline samples. At low temperatures, a quasielastic magnetic response with a half-width Gamma approximate to 0.1 meV persists with varying intensity all over the Brillouin zone. It forms a broad hump centered at the (111) scattering vector, surrounded by minima of intensity at (002), (220), and equivalent wave vectors. The momentum-space structure distinguishes this signal from a simple crystal-field excitation at 0.31 meV, suggested previously, and rather lets us ascribe it to short-range dynamical correlations between the neighboring Ce ions, mediated by the itinerant heavy f electrons via the Ruderman-Kittel-Kasuya-Yosida mechanism. With increasing temperature, the energy width of the signal follows the conventional T-1/2 law, Gamma(T) = Gamma(0) + A root T. The momentum-space symmetry of the quasielastic response suggests that it stems from the simple-cubic Ce sublattice occupying the 8c Wyckoff site, whereas the crystallographically inequivalent 4a site remains magnetically silent in this material. C1 [Portnichenko, P. Y.; Cameron, A. S.; Surmach, M. A.; Inosov, D. S.] Tech Univ Dresden, Inst Festkorperphys, D-01069 Dresden, Germany. [Deen, P. P.] European Spallat Source ESS AB, SE-22100 Lund, Sweden. [Deen, P. P.] Univ Copenhagen, Niels Bohr Inst, DK-2100 Copenhagen, Denmark. [Paschen, S.; Prokofiev, A.] Vienna Univ Technol, Inst Solid State Phys, A-1040 Vienna, Austria. [Mignot, J. -M.] CEA Saclay, CEA CNRS, Lab Leon Brillouin, F-91191 Gif Sur Yvette, France. [Strydom, A. M.] Univ Johannesburg, Dept Phys, ZA-2006 Auckland Pk, South Africa. [Telling, M. T. F.] Rutherford Appleton Lab, ISIS Facil, Didcot OX1 10QX, Oxon, England. [Telling, M. T. F.] Univ Oxford, Dept Mat, Oxford OX1 3PH, England. [Podlesnyak, A.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. RP Inosov, DS (reprint author), Tech Univ Dresden, Inst Festkorperphys, D-01069 Dresden, Germany. EM Dmytro.Inosov@tu-dresden.de RI Instrument, CNCS/B-4599-2012; Podlesnyak, Andrey/A-5593-2013; Inosov, Dmytro/B-6781-2008; Mignot, Jean-Michel/A-8305-2008; Telling, Mark/F-3294-2014; OI Podlesnyak, Andrey/0000-0001-9366-6319; Mignot, Jean-Michel/0000-0001-8503-6712; Paschen, Silke/0000-0002-3796-0713 FU German Research Foundation (DFG) [IN 209/3-1]; European Research Council [227378]; European Commission [283883]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; Research Training Group GRK 1621 at the TUDresden FX We are grateful to P. Boutrouille (LLB) and S. Elorfi (SNS) for technical support during the experiments. Reduction of the TOF data was performed using the HORACE software package [39]. This project was funded by the German Research Foundation (DFG) under Grant No. IN 209/3-1 and via the Research Training Group GRK 1621 at the TUDresden, by the European Research Council (Advanced Grant QuantumPuzzle, Grant No. 227378), and by the European Commission under the 7th Framework Programme NMI3-II/FP7-Contract No. 283883. Research at Oak Ridge National Laboratory's Spallation Neutron Source was supported by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. NR 40 TC 5 Z9 5 U1 3 U2 30 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAR 13 PY 2015 VL 91 IS 9 AR 094412 DI 10.1103/PhysRevB.91.094412 PG 6 WC Physics, Condensed Matter SC Physics GA CD9QB UT WOS:000351431800001 ER PT J AU Kizilersu, A Sizer, T Pennington, MR Williams, AG Williams, R AF Kizilersue, Ayse Sizer, Tom Pennington, Michael R. Williams, Anthony G. Williams, Richard TI Dynamical mass generation in unquenched QED using the Dyson-Schwinger equations SO PHYSICAL REVIEW D LA English DT Article ID CHIRAL-SYMMETRY-BREAKING; RENORMALIZATION-GROUP FLOW; GAUGE FIELD-THEORIES; QUANTUM ELECTRODYNAMICS; PHASE-TRANSITION; CONTINUUM-LIMIT; 4-FERMION INTERACTION; CRITICAL EXPONENTS; COVARIANT GAUGES; WARD IDENTITY AB We present a comprehensive numerical study of dynamical mass generation for unquenched QED in four dimensions, in the absence of four-fermion interactions, using the Dyson-Schwinger approach. We begin with an overview of previous investigations of criticality in the quenched approximation. To this we add an analysis using a new fermion-antifermion-boson interaction ansatz, the Kizilersu-Pennington (KP) vertex, developed for an unquenched treatment. After surveying criticality in previous unquenched studies, we investigate the performance of the KP vertex in dynamical mass generation using a renormalized fully unquenched system of equations. This we compare with the results for two hybrid vertices incorporating the Curtis-Pennington vertex in the fermion equation. We conclude that the KP vertex is as yet incomplete, and its relative gauge variance is due to its lack of massive transverse components in its design. C1 [Kizilersue, Ayse; Sizer, Tom; Williams, Anthony G.] Univ Adelaide, Dept Phys, Special Res Ctr Subat Struct Matter, Adelaide, SA 5005, Australia. [Pennington, Michael R.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. [Williams, Anthony G.] Univ Adelaide, Sch Chem & Phys, ARC Ctr Excellence Particle Phys Terascale, Adelaide, SA 5005, Australia. [Williams, Richard] Univ Giessen, Inst Theoret Phys, D-35392 Giessen, Germany. RP Kizilersu, A (reprint author), Univ Adelaide, Dept Phys, Special Res Ctr Subat Struct Matter, Adelaide, SA 5005, Australia. EM akiziler@physics.adelaide.edu.au; tsizer@physics.adelaide.edu.au; michaelp@jlab.org; anthony.williams@adelaide.edu.au; richard.williams@theo.physik.uni-giessen.de OI Williams, Anthony/0000-0002-1472-1592 FU Australian Research Council International Linkage Award [LX 0776452]; Austrian Science Fund (FWF) [M1333-N16]; Jefferson Science Associates, LLC under U.S. DOE [DE-AC05-06OR23177]; Centre for the Subatomic Structure of Matter (CSSM); Australian Research Council Discovery [DP0558878] FX We would like to thank C. S. Fischer and C. D. Roberts for useful discussions. A. K. and T. S. thank A. W. Thomas for supporting this study under the aegis of the Centre for the Subatomic Structure of Matter (CSSM). We also acknowledge support from the Australian Research Council International Linkage Award (No. LX 0776452), the Australian Research Council Discovery grant (No. DP0558878), and the Austrian Science Fund (FWF) under Project No. M1333-N16. M. R. P. acknowledges support of Jefferson Science Associates, LLC under U.S. DOE Contract No. DE-AC05-06OR23177 for the writing of this paper. NR 95 TC 3 Z9 3 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 13 PY 2015 VL 91 IS 6 AR 065015 DI 10.1103/PhysRevD.91.065015 PG 17 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CD9QP UT WOS:000351433200010 ER PT J AU Berger, RL Suter, LJ Divol, L London, RA Chapman, T Froula, DH Meezan, NB Neumayer, P Glenzer, SH AF Berger, R. L. Suter, L. J. Divol, L. London, R. A. Chapman, T. Froula, D. H. Meezan, N. B. Neumayer, P. Glenzer, S. H. TI Beyond the gain exponent: Effect of damping, scale length, and speckle length on stimulated scatter SO PHYSICAL REVIEW E LA English DT Article ID NATIONAL-IGNITION-FACILITY; LASER PERFORMANCE; PLASMAS; WAVES; BEAMS AB Three-dimensional wave propagation simulations and experiments show that the gain exponent, an often used metric to assess the likelihood of stimulated Brillouin scatter, is insufficient and must be augmented with another parameter, N-r, the ratio of the resonance length, L-res, to the laser speckle length. The damping rate of ion acoustic waves, nu, and thus L-res, which is proportional to nu, are easily varied with plasma species composition, e.g., by varying the ratio of hydrogen and carbon ions. As N-r decreases, stimulated Brillouin scattering increases despite the same gain exponent. C1 [Berger, R. L.; Suter, L. J.; Divol, L.; London, R. A.; Chapman, T.; Meezan, N. B.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Froula, D. H.] Univ Rochester, Laser Energet Lab, New York, NY 14623 USA. [Neumayer, P.] GSI Helmholtzzentrum Schwerionenforsch, ExtreMe Matter Inst EMMI, D-64291 Darmstadt, Germany. [Glenzer, S. H.] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. RP Berger, RL (reprint author), Lawrence Livermore Natl Lab, POB 808, Livermore, CA 94551 USA. EM berger5@llnl.gov FU US Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX We are pleased to acknowledge stimulating discussions with E. A. Williams, D. J. Strozzi, C. H. Still, P. Michel, A. B. Langdon, and D. E. Hinkel. We also wish to express our appreciation to M. R. Dorr for developing the methods for incorporating plasma parameters from hydrodynamic simulation into pF3D simulations, and to J. A. Hittinger for developing the multifluid hydrodynamics in pF3D without which our numerous pF3D simulations of NIF and OMEGA experiments in the last decade would not be possible. This work was performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 23 TC 1 Z9 1 U1 1 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1539-3755 EI 1550-2376 J9 PHYS REV E JI Phys. Rev. E PD MAR 13 PY 2015 VL 91 IS 3 AR 031103 DI 10.1103/PhysRevE.91.031103 PG 5 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA CD9QR UT WOS:000351433400002 PM 25871045 ER PT J AU Bulanov, SS Esarey, E Schroeder, CB Bulanov, SV Esirkepov, TZ Kando, M Pegoraro, F Leemans, WP AF Bulanov, S. S. Esarey, E. Schroeder, C. B. Bulanov, S. V. Esirkepov, T. Zh. Kando, M. Pegoraro, F. Leemans, W. P. TI Enhancement of Maximum Attainable Ion Energy in the Radiation Pressure Acceleration Regime Using a Guiding Structure SO PHYSICAL REVIEW LETTERS LA English DT Article ID INTENSE LASER-PULSES; ULTRA-INTENSE; UNDERDENSE PLASMA; FAST IGNITION; ELECTRODYNAMICS; GENERATION; PHYSICS AB Radiation pressure acceleration is a highly efficient mechanism of laser-driven ion acceleration, with the laser energy almost totally transferrable to the ions in the relativistic regime. There is a fundamental limit on the maximum attainable ion energy, which is determined by the group velocity of the laser. In the case of tightly focused laser pulses, which are utilized to get the highest intensity, another factor limiting the maximum ion energy comes into play, the transverse expansion of the target. Transverse expansion makes the target transparent for radiation, thus reducing the effectiveness of acceleration. Utilization of an external guiding structure for the accelerating laser pulse may provide a way of compensating for the group velocity and transverse expansion effects. C1 [Bulanov, S. S.; Leemans, W. P.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Esarey, E.; Schroeder, C. B.; Leemans, W. P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Bulanov, S. V.; Esirkepov, T. Zh.; Kando, M.] JAEA, Kansai Photon Sci Inst, Kizugawa, Kyoto 6190215, Japan. [Bulanov, S. V.] Russian Acad Sci, Prokhorov Inst Gen Phys, Moscow 119991, Russia. [Bulanov, S. V.] Moscow Inst Phys & Technol, Dolgoprudnyi 141700, Moscow Region, Russia. [Pegoraro, F.] Univ Pisa, Dept Phys, I-56127 Pisa, Italy. [Pegoraro, F.] CNR, Ist Nazl Ott, I-56127 Pisa, Italy. RP Bulanov, SS (reprint author), Univ Calif Berkeley, Berkeley, CA 94720 USA. RI Bulanov, Sergei/A-1721-2013; OI Schroeder, Carl/0000-0002-9610-0166 FU NSF [PHY-0935197]; Office of Science of the US DOE [DE-AC02-05CH11231, DE-FG02-12ER41798]; Ministry of Education, Youth, and Sports of the Czech Republic [CZ.1.05/1.1.00/02.0061] FX We acknowledge support from the NSF under Grant No. PHY-0935197 and the Office of Science of the US DOE under Contracts No. DE-AC02-05CH11231 and No. DE-FG02-12ER41798 and Ministry of Education, Youth, and Sports of the Czech Republic under the Project No. CZ.1.05/1.1.00/02.0061. The authors would like to thank C. Benedetti, M. Chen, C. G. R. Geddes, and L. Yu for discussions. NR 43 TC 8 Z9 8 U1 4 U2 39 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 13 PY 2015 VL 114 IS 10 AR 105003 DI 10.1103/PhysRevLett.114.105003 PG 5 WC Physics, Multidisciplinary SC Physics GA CD9QS UT WOS:000351433500005 PM 25815939 ER PT J AU Luo, L Chatzakis, I Patz, A Wang, JG AF Luo, Liang Chatzakis, Ioannis Patz, Aaron Wang, Jigang TI Ultrafast Terahertz Probes of Interacting Dark Excitons in Chirality-Specific Semiconducting Single-Walled Carbon Nanotubes SO PHYSICAL REVIEW LETTERS LA English DT Article ID ABSORPTION AB Ultrafast terahertz spectroscopy accesses the dark excitonic ground state in resonantly excited (6,5) single-walled carbon nanotubes via internal, direct dipole-allowed transitions between the lowest-lying dark-bright pair state of similar to 6 meV. An analytical model reproduces the response that enables the quantitative analysis of transient densities of dark excitons and e-h plasma, oscillator strength, transition energy renormalization, and dynamics. Nonequilibrium, yet stable, quasi-one-dimensional quantum states with dark excitonic correlations rapidly emerge even with increasing off-resonance photoexcitation and experience a unique crossover to complex phase-space filling of both dark and bright pair states, different from dense two-and three-dimensional excitons influenced by the thermalization, cooling, and ionization to free carriers. C1 [Wang, Jigang] Iowa State Univ, Dept Phys & Astron, US DOE, Ames, IA 50011 USA. Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. RP Wang, JG (reprint author), Iowa State Univ, Dept Phys & Astron, US DOE, Ames, IA 50011 USA. EM jgwang@iastate.edu FU U.S. Department of Energy, Office of Basic Energy Science, Division of Materials Sciences and Engineering [DE-AC02-07CH11358] FX This work was supported by the U.S. Department of Energy, Office of Basic Energy Science, Division of Materials Sciences and Engineering (Ames Laboratory is operated for the U.S. Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358). NR 36 TC 9 Z9 9 U1 3 U2 38 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 13 PY 2015 VL 114 IS 10 AR 107402 DI 10.1103/PhysRevLett.114.107402 PG 5 WC Physics, Multidisciplinary SC Physics GA CD9QS UT WOS:000351433500009 PM 25815965 ER PT J AU McMinis, J Clay, RC Lee, D Morales, MA AF McMinis, Jeremy Clay, Raymond C., III Lee, Donghwa Morales, Miguel A. TI Molecular to Atomic Phase Transition in Hydrogen under High Pressure SO PHYSICAL REVIEW LETTERS LA English DT Article ID SOLID HYDROGEN; MEGABAR PRESSURES; METALLIC HYDROGEN; DENSE HYDROGEN; SIMULATIONS; FLUID AB The metallization of high-pressure hydrogen, together with the associated molecular to atomic transition, is one of the most important problems in the field of high-pressure physics. It is also currently a matter of intense debate due to the existence of conflicting experimental reports on the observation of metallic hydrogen on a diamond-anvil cell. Theoretical calculations have typically relied on a mean-field description of electronic correlation through density functional theory, a theory with well-known limitations in the description of metal-insulator transitions. In fact, the predictions of the pressure-driven dissociation of molecules in high-pressure hydrogen by density functional theory is strongly affected by the chosen exchange-correlation functional. In this Letter, we use quantum Monte Carlo calculations to study the molecular to atomic transition in hydrogen. We obtain a transition pressure of 447(3) GPa, in excellent agreement with the best experimental estimate of the transition 450 GPa based on an extrapolation to zero band gap from experimental measurements. Additionally, we find that C2/c is stable almost up to the molecular to atomic transition, in contrast to previous density functional theory (DFT) and DFT + quantum Monte Carlo studies which predict large stability regimes for intermediary molecular phases. C1 [McMinis, Jeremy; Clay, Raymond C., III; Lee, Donghwa; Morales, Miguel A.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Clay, Raymond C., III] Univ Illinois, Urbana, IL 61821 USA. RP Morales, MA (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM moralessilva2@llnl.gov FU U.S. Department of Energy at the Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Laboratory Directed Research and Development [13-LW-004] FX This work was supported by the U.S. Department of Energy at the Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344 and by Laboratory Directed Research and Development Grant No. 13-LW-004. Computer resources have been provided by Lawrence Livermore National Laboratory through the 7th Institutional Unclassified Computing Grand Challenge program. NR 49 TC 10 Z9 10 U1 7 U2 44 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 13 PY 2015 VL 114 IS 10 AR 105305 DI 10.1103/PhysRevLett.114.105305 PG 6 WC Physics, Multidisciplinary SC Physics GA CD9QS UT WOS:000351433500006 PM 25815944 ER PT J AU Huang, XJ Lauer, K Clark, JN Xu, WH Nazaretski, E Harder, R Robinson, IK Chu, YS AF Huang, Xiaojing Lauer, Kenneth Clark, Jesse N. Xu, Weihe Nazaretski, Evgeny Harder, Ross Robinson, Ian K. Chu, Yong S. TI Fly-scan ptychography SO SCIENTIFIC REPORTS LA English DT Article ID WIGNER-DISTRIBUTION DECONVOLUTION; K-B MIRRORS; PHASE-RETRIEVAL; COMPUTED-TOMOGRAPHY; ELECTRON-MICROSCOPY; RAY; DIFFRACTION; RESOLUTION; OPTIMIZATION; NANOSCALE AB We report an experimental ptychography measurement performed in fly-scan mode. With a visible-light laser source, we demonstrate a 5-fold reduction of data acquisition time. By including multiple mutually incoherent modes into the incident illumination, high quality images were successfully reconstructed from blurry diffraction patterns. This approach significantly increases the throughput of ptychography, especially for three-dimensional applications and the visualization of dynamic systems. C1 [Huang, Xiaojing; Lauer, Kenneth; Xu, Weihe; Nazaretski, Evgeny; Chu, Yong S.] Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA. [Clark, Jesse N.] SLAC, Stanford PULSE Inst, Natl Accelerator Lab, Menlo Pk, CA 94205 USA. [Clark, Jesse N.] Deutsch Elektronensynchrotron, Ctr Free Elect Laser Sci, D-22607 Hamburg, Germany. [Harder, Ross] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Robinson, Ian K.] UCL, London Ctr Nanotechnol, London WC1H 0AH, England. [Robinson, Ian K.] Res Complex Harwell, Didcot OX11 0DE, Oxon, England. RP Huang, XJ (reprint author), Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA. EM xjhuang@bnl.gov RI Huang, Xiaojing/K-3075-2012 OI Huang, Xiaojing/0000-0001-6034-5893 FU Department of Energy, Office of Basic Energy Sciences [DE-AC-02-98CH10886]; ERC "nanosculpture" [227711]; Volkswagen Foundation FX Work at Brookhaven was supported by the Department of Energy, Office of Basic Energy Sciences under contract DE-AC-02-98CH10886. I.K.R. is supported by the ERC "nanosculpture" advanced grant 227711. J.N.C. gratefully acknowledges financial support from the Volkswagen Foundation. NR 43 TC 6 Z9 7 U1 4 U2 27 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAR 13 PY 2015 VL 5 AR 9074 DI 10.1038/srep09074 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CD5SY UT WOS:000351149500005 PM 25766519 ER PT J AU Martinez, E Uberuaga, BP AF Martinez, Enrique Uberuaga, Blas P. TI Mobility and coalescence of stacking fault tetrahedra in Cu SO SCIENTIFIC REPORTS LA English DT Article ID QUENCHED GOLD; DISLOCATION DYNAMICS; DIPOLE ANNIHILATION; ENERGY CALCULATIONS; IRRADIATED COPPER; VACANCY CLUSTERS; AL; GROWTH; SIMULATION; STRENGTH AB Stacking fault tetrahedra (SFTs) are ubiquitous defects in face-centered cubic metals. They are produced during cold work plastic deformation, quenching experiments or under irradiation. From a dislocation point of view, the SFTs are comprised of a set of stair-rod dislocations at the (110) edges of a tetrahedron bounding triangular stacking faults. These defects are extremely stable, increasing their energetic stability as they grow in size. At the sizes visible within transmission electron microscope they appear nearly immobile. Contrary to common belief, we show in this report, using a combination of molecular dynamics and temperature accelerated dynamics, how small SFTs can diffuse by temporarily disrupting their structure through activated thermal events. More over, we demonstrate that the diffusivity of defective SFTs is several orders of magnitude higher than perfect SFTs, and can be even higher than isolated vacancies. Finally, we show how SFTs can coalesce, forming a larger defect in what is a new mechanism for the growth of these omnipresent defects. C1 [Martinez, Enrique; Uberuaga, Blas P.] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. RP Martinez, E (reprint author), Los Alamos Natl Lab, Div Mat Sci & Technol, MST 8, Los Alamos, NM 87545 USA. EM enriquem@lanl.gov OI Martinez Saez, Enrique/0000-0002-2690-2622 FU US Department of Energy (DOE); U.S. DOE [DE-AC52-06NA25396] FX The authors gratefully acknowledge the support of the US Department of Energy (DOE) through the LANL/LDRD Program for this work. This research used resources provided by the LANL Institutional Computing Program. LANL, an affirmative action/equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. DOE under contract DE-AC52-06NA25396. NR 33 TC 6 Z9 6 U1 9 U2 40 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAR 13 PY 2015 VL 5 AR 9084 DI 10.1038/srep09084 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CD5SY UT WOS:000351149500015 PM 25765711 ER PT J AU Jain, P Wang, Q Roldan, M Glavic, A Lauter, V Urban, C Bi, Z Ahmed, T Zhu, J Varela, M Jia, QX Fitzsimmons, MR AF Jain, P. Wang, Q. Roldan, M. Glavic, A. Lauter, V. Urban, C. Bi, Z. Ahmed, T. Zhu, J. Varela, M. Jia, Q. X. Fitzsimmons, M. R. TI Synthetic magnetoelectric coupling in a nanocomposite multiferroic SO SCIENTIFIC REPORTS LA English DT Article ID THIN-FILM HETEROSTRUCTURES; EXCHANGE BIAS; ELECTRIC CONTROL; BIFEO3 AB Given the paucity of single phase multiferroic materials (with large ferromagnetic moment), composite systems seem an attractive solution to realize magnetoelectric coupling between ferromagnetic and ferroelectric order parameters. Despite having antiferromagnetic order, BiFeO3 (BFO) has nevertheless been a key material due to excellent ferroelectric properties at room temperature. We studied a superlattice composed of 8 repetitions of 6 unit cells of La0.7Sr0.3MnO3 (LSMO) grown on 5 unit cells of BFO. Significant net uncompensated magnetization in BFO, an insulating superlattice, is demonstrated using polarized neutron reflectometry. Remarkably, the magnetization enables magnetic field to change the dielectric properties of the superlattice, which we cite as an example of synthetic magnetoelectric coupling. Importantly, controlled creation of magnetic moment in BFO is a much needed path toward design and implementation of integrated oxide devices for next generation magnetoelectric data storage platforms. C1 [Jain, P.; Wang, Q.; Bi, Z.; Ahmed, T.; Zhu, J.; Jia, Q. X.; Fitzsimmons, M. R.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Roldan, M.; Varela, M.] Univ Complutense Madrid, E-28040 Madrid, Spain. [Glavic, A.; Lauter, V.; Varela, M.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Urban, C.] Univ Calif San Diego, La Jolla, CA 92093 USA. RP Fitzsimmons, MR (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM fitzsimmonsm@ornl.gov RI Varela, Maria/E-2472-2014; Glavic, Artur/B-3453-2015 OI Varela, Maria/0000-0002-6582-7004; Glavic, Artur/0000-0003-4951-235X FU LANL/LDRD program; U.S. Department of Energy (DOE) Office of Science; Scientific User Facilities Division of the Department of Energy's Office of Basic Energy Science; Los Alamos National Security LLC under DOE [DE-AC52-06NA25396]; U.S. National Science Foundation I2CAM International Materials Institute Award [DMR-1411344]; Office of Basic Energy Science, U.S. Department of Energy, BES DMS - Department of Energy's Office of Basic Energy Science, DMR [DE FG02 87ER-45332]; ERC Starting Investigator Award STEMOX [739239]; [NSF-DMR-1157490] FX This work was supported by the LANL/LDRD program and was performed, in part, at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science. This work has benefited from the use of the Spallation Neutron Source (Oak Ridge National Laboratory) and the Lujan Neutron Scattering Center (Los Alamos National Laboratory), which are funded by the Scientific User Facilities Division of the Department of Energy's Office of Basic Energy Science. Part of the work was carried out at the National High Magnetic Field Laboratory's High B/T Facility supported by the NSF-DMR-1157490. Los Alamos National Laboratory is operated by Los Alamos National Security LLC under DOE Contract DE-AC52-06NA25396. P.J. would also like to acknowledge the support of the U.S. National Science Foundation I2CAM International Materials Institute Award, Grant DMR-1411344. The research at UCSD was supported by the Office of Basic Energy Science, U.S. Department of Energy, BES DMS funded by the Department of Energy's Office of Basic Energy Science, DMR under grant DE FG02 87ER-45332. Research at UCM sponsored by the ERC Starting Investigator Award STEMOX 739239. NR 21 TC 8 Z9 8 U1 8 U2 101 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAR 13 PY 2015 VL 5 AR 9089 DI 10.1038/srep09089 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CD5TG UT WOS:000351150300002 PM 25766205 ER PT J AU Uberuaga, BP Vernon, LJ Martinez, E Voter, AF AF Uberuaga, Blas Pedro Vernon, Louis J. Martinez, Enrique Voter, Arthur F. TI The relationship between grain boundary structure, defect mobility, and grain boundary sink efficiency SO SCIENTIFIC REPORTS LA English DT Article ID COMPUTER-SIMULATION; MOLECULAR-DYNAMICS; VACANCY MECHANISM; SELF-DIFFUSION; DISLOCATIONS; INTERFACES; METALS; CU; IMPURITIES; RADIATION AB Nanocrystalline materials have received great attention due to their potential for improved functionality and have been proposed for extreme environments where the interfaces are expected to promote radiation tolerance. However, the precise role of the interfaces in modifying defect behavior is unclear. Using long-time simulations methods, we determine the mobility of defects and defect clusters at grain boundaries in Cu. We find thatmobilities vary significantly with boundary structure and cluster size, with larger clusters exhibiting reduced mobility, and that interface sink efficiency depends on the kinetics of defects within the interface via the in-boundary annihilation rate of defects. Thus, sink efficiency is a strong function of defect mobility, which depends on boundary structure, a property that evolves with time. Further, defect mobility at boundaries can be slower than in the bulk, which has general implications for the properties of polycrystalline materials. Finally, we correlate defect energetics with the volumes of atomic sites at the boundary. C1 [Uberuaga, Blas Pedro; Martinez, Enrique] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. [Vernon, Louis J.] Los Alamos Natl Lab, Comp Computat & Stat Sci Div, Los Alamos, NM 87545 USA. [Voter, Arthur F.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Uberuaga, BP (reprint author), Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. EM blas@lanl.gov OI Martinez Saez, Enrique/0000-0002-2690-2622; Vernon, Louis/0000-0001-5379-7488 FU Center for Materials at Irradiation and Mechanical Extremes; Energy Frontier Research Center - U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences (BES) [2008LANL1026]; BES, Materials Science and Engineering Division; National Nuclear Security Administration of the U.S. DOE [DE-AC52-06NA25396] FX This work was supported as part of the Center for Materials at Irradiation and Mechanical Extremes, an Energy Frontier Research Center funded by the U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences (BES) under Award Number 2008LANL1026. AFV acknowledges support from BES, Materials Science and Engineering Division. Los Alamos National Laboratory, an affirmative action equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. DOE under contract DE-AC52-06NA25396. NR 50 TC 25 Z9 25 U1 4 U2 46 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAR 13 PY 2015 VL 5 AR 9095 DI 10.1038/srep09095 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CD5TG UT WOS:000351150300008 PM 25766999 ER PT J AU Olama, MM Ma, X Killough, SM Kuruganti, T Smith, SF Djouadi, SM AF Olama, Mohammed M. Ma, Xiao Killough, Stephen M. Kuruganti, Teja Smith, Stephen F. Djouadi, Seddik M. TI Analysis, optimization, and implementation of a hybrid DS/FFH spread-spectrum technique for smart grid communications SO EURASIP JOURNAL ON ADVANCES IN SIGNAL PROCESSING LA English DT Article DE Hybrid spread-spectrum; Direct sequence; Frequency hopping; Smart grid communications; Non-convex optimization; Receiver sensitivity; FPGA ID MULTIPLE-ACCESS COMMUNICATIONS; RICIAN-FADING CHANNELS; ERROR-PROBABILITY; SEQUENCE; MODULATION; SYSTEMS AB In recent years, there has been great interest in using hybrid spread-spectrum (HSS) techniques for commercial applications, particularly in the Smart Grid, in addition to their inherent uses in military communications. This is because HSS can accommodate high data rates with high link integrity, even in the presence of significant multipath effects and interfering signals. A highly useful form of this transmission technique for many types of command, control, and sensing applications is the specific code-related combination of standard direct sequence modulation with 'fast' frequency hopping, denoted hybrid DS/FFH, wherein multiple frequency hops occur within a single data-bit time. In this paper, error-probability analyses are performed for a hybrid DS/FFH system over standard Gaussian and fading-type channels, progressively including the effects from wide-and partial-band jamming, multi-user interference, and varying degrees of Rayleigh and Rician fading. In addition, an optimization approach is formulated that minimizes the bit-error performance of a hybrid DS/FFH communication system and solves for the resulting system design parameters. The optimization objective function is non-convex and can be solved by applying the Karush-Kuhn-Tucker conditions. We also present our efforts toward exploring the design, implementation, and evaluation of a hybrid DS/FFH radio transceiver using a single field-programmable gate array (FPGA). Numerical and experimental results are presented under widely varying design parameters to demonstrate the adaptability of the waveform for varied harsh smart grid RF signal environments. C1 [Olama, Mohammed M.; Killough, Stephen M.; Kuruganti, Teja; Smith, Stephen F.] Oak Ridge Natl Lab, Computat Sci & Engn Div, Oak Ridge, TN 37831 USA. [Ma, Xiao; Djouadi, Seddik M.] Univ Tennessee, Dept Elect Engn & Comp Sci, Knoxville, TN 37996 USA. [Djouadi, Seddik M.] Masdar Inst Sci & Technol, Dept Elect Engn & Comp Sci, Abu Dhabi, U Arab Emirates. RP Olama, MM (reprint author), Oak Ridge Natl Lab, Computat Sci & Engn Div, POB 2008,MS 6085, Oak Ridge, TN 37831 USA. EM olamahussemm@ornl.gov FU U.S. Department of Energy [DE-AC05-00OR22725]; DOE Public Access Plan; NSF [CMMI-1334094] FX This manuscript has been authored by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan. In addition, this work has been partially supported by NSF grant CMMI-1334094. NR 28 TC 1 Z9 1 U1 0 U2 7 PU SPRINGER INTERNATIONAL PUBLISHING AG PI CHAM PA GEWERBESTRASSE 11, CHAM, CH-6330, SWITZERLAND SN 1687-6180 J9 EURASIP J ADV SIG PR JI EURASIP J. Adv. Signal Process. PD MAR 12 PY 2015 AR 25 DI 10.1186/s13634-015-0208-z PG 18 WC Engineering, Electrical & Electronic SC Engineering GA CE8OF UT WOS:000352101900001 ER PT J AU Biswal, AK Hao, ZY Pattathil, S Yang, XH Winkeler, K Collins, C Mohanty, SS Richardson, EA Gelineo-Albersheim, I Hunt, K Ryno, D Sykes, RW Turner, GB Ziebell, A Gjersing, E Lukowitz, WG Davis, MF Decker, SR Hahn, MG Mohnen, D AF Biswal, Ajaya K. Hao, Zhangying Pattathil, Sivakumar Yang, Xiaohan Winkeler, Kim Collins, Cassandra Mohanty, Sushree S. Richardson, Elizabeth A. Gelineo-Albersheim, Ivana Hunt, Kimberly Ryno, David Sykes, Robert W. Turner, Geoffrey B. Ziebell, Angela Gjersing, Erica Lukowitz, Wolfgang Davis, Mark F. Decker, Stephen R. Hahn, Michael G. Mohnen, Debra TI Downregulation of GAUT12 in Populus deltoides by RNA silencing results in reduced recalcitrance, increased growth and reduced xylan and pectin in a woody biofuel feedstock SO BIOTECHNOLOGY FOR BIOFUELS LA English DT Article DE Biofuel; Growth; Pectin; Populus; Saccharification; Secondary cell wall; Xylan; Wood development ID SECONDARY CELL-WALL; BIOSYNTHETIC HOMOGALACTURONAN GALACTURONOSYLTRANSFERASE; AGROBACTERIUM-MEDIATED TRANSFORMATION; GLYCOSYLTRANSFERASE FAMILY 8; GLUCURONOXYLAN BIOSYNTHESIS; ARABIDOPSIS-THALIANA; MOLECULAR CHARACTERIZATION; IMPROVES SACCHARIFICATION; GENETICS ANALYSIS; MUTANTS REVEALS AB Background: The inherent recalcitrance of woody bioenergy feedstocks is a major challenge for their use as a source of second-generation biofuel. Secondary cell walls that constitute the majority of hardwood biomass are rich in cellulose, xylan, and lignin. The interactions among these polymers prevent facile accessibility and deconstruction by enzymes and chemicals. Plant biomass that can with minimal pretreatment be degraded into sugars is required to produce renewable biofuels in a cost-effective manner. Results: GAUT12/IRX8 is a putative glycosyltransferase proposed to be involved in secondary cell wall glucuronoxylan and/or pectin biosynthesis based on concomitant reductions of both xylan and the pectin homogalacturonan (HG) in Arabidopsis irx8 mutants. Two GAUT12 homologs exist in Populus trichocarpa, PtGAUT12.1 and PtGAUT12.2. Knockdown expression of both genes simultaneously has been shown to reduce xylan content in Populus wood. We tested the proposition that RNA interference (RNAi) downregulation of GAUT12.1 alone would lead to increased sugar release in Populus wood, that is, reduced recalcitrance, based on the hypothesis that GAUT12 synthesizes a wall structure required for deposition of xylan and that cell walls with less xylan and/or modified cell wall architecture would have reduced recalcitrance. Using an RNAi approach, we generated 11 Populus deltoides transgenic lines with 50 to 67% reduced PdGAUT12.1 transcript expression compared to wild type (WT) and vector controls. Ten of the eleven RNAi lines yielded 4 to 8% greater glucose release upon enzymatic saccharification than the controls. The PdGAUT12.1 knockdown (PdGAUT12.1-KD) lines also displayed 12 to 52% and 12 to 44% increased plant height and radial stem diameter, respectively, compared to the controls. Knockdown of PdGAUT12.1 resulted in a 25 to 47% reduction in galacturonic acid and 17 to 30% reduction in xylose without affecting total lignin content, revealing that in Populus wood as in Arabidopsis, GAUT12 affects both pectin and xylan formation. Analyses of the sugars present in sequential cell wall extracts revealed a reduction of glucuronoxylan and pectic HG and rhamnogalacturonan in extracts from PdGAUT12.1-KD lines. Conclusions: The results show that downregulation of GAUT12.1 leads to a reduction in a population of xylan and pectin during wood formation and to reduced recalcitrance, more easily extractable cell walls, and increased growth in Populus. C1 [Biswal, Ajaya K.; Mohnen, Debra] Univ Georgia, Dept Biochem & Mol Biol, Athens, GA 30602 USA. [Hao, Zhangying; Richardson, Elizabeth A.; Lukowitz, Wolfgang; Hahn, Michael G.] Univ Georgia, Dept Plant Biol, Athens, GA 30602 USA. [Biswal, Ajaya K.; Hao, Zhangying; Pattathil, Sivakumar; Mohanty, Sushree S.; Gelineo-Albersheim, Ivana; Hunt, Kimberly; Ryno, David; Hahn, Michael G.; Mohnen, Debra] Univ Georgia, Complex Carbohydrate Res Ctr, Athens, GA 30602 USA. [Biswal, Ajaya K.; Hao, Zhangying; Pattathil, Sivakumar; Yang, Xiaohan; Winkeler, Kim; Collins, Cassandra; Mohanty, Sushree S.; Gelineo-Albersheim, Ivana; Hunt, Kimberly; Ryno, David; Sykes, Robert W.; Turner, Geoffrey B.; Ziebell, Angela; Gjersing, Erica; Davis, Mark F.; Decker, Stephen R.; Hahn, Michael G.; Mohnen, Debra] DOE BioEnergy Sci Ctr BESC, Oak Ridge, TN USA. [Yang, Xiaohan] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. [Winkeler, Kim; Collins, Cassandra] ArborGen Inc, Ridgeville, SC 29472 USA. [Sykes, Robert W.; Turner, Geoffrey B.; Ziebell, Angela; Gjersing, Erica; Davis, Mark F.; Decker, Stephen R.] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Mohnen, D (reprint author), Univ Georgia, Dept Biochem & Mol Biol, B122 Life Sci Bldg, Athens, GA 30602 USA. EM dmohnen@ccrc.uga.edu RI Yang, Xiaohan/A-6975-2011; OI Yang, Xiaohan/0000-0001-5207-4210; , Sivakumar Pattathil/0000-0003-3870-4137; davis, mark/0000-0003-4541-9852 FU US National Science Foundation Plant Genome Program [DBI-0421683, IOS-0923992]; BioEnergy Science Center (BESC) [DE-PS02-06ER64304]; Department of Energy Center [DE-FG02-93ER20097]; Office of Biological and Environmental Research in the DOE Office of Science FX We thank Lee Gunter for validation of constructs containing amplified gene targets from P. trichocarpa leaf cDNA libraries, Rick Nelson for directing the BESC transformation pipeline and critical review of the manuscript, Will Rottmann for overseeing the Populus transformation pipeline, Sheilah Dixon Huckabee for administrative assistance, and the CCRC Analytical Services for glycosyl residue linkage analysis. The authors also thank Crissa Doeppke, Melissa Glenn, Kimberly Mazza, Logan Schuster, and Kevin Cowley for preparation of samples for the HTP biomass recalcitrance pipeline and Breeanna R. Urbanowicz for providing the poplar cDNA. The generation of the CCRC series of plant cell wall glycan-directed monoclonal antibodies used in this work was supported by the US National Science Foundation Plant Genome Program (DBI-0421683 and IOS-0923992). The research was funded by The BioEnergy Science Center (BESC) Grant DE-PS02-06ER64304 and partially by the Department of Energy Center Grant DE-FG02-93ER20097. The BioEnergy Science Center is a U.S. Department of Energy Bioenergy Research Center supported by the Office of Biological and Environmental Research in the DOE Office of Science. NR 74 TC 11 Z9 11 U1 5 U2 41 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1754-6834 J9 BIOTECHNOL BIOFUELS JI Biotechnol. Biofuels PD MAR 12 PY 2015 VL 8 AR 41 DI 10.1186/s13068-015-0218-y PG 25 WC Biotechnology & Applied Microbiology; Energy & Fuels SC Biotechnology & Applied Microbiology; Energy & Fuels GA CE5UK UT WOS:000351901000001 PM 25802552 ER PT J AU Payne, CE Wolfrum, EJ AF Payne, Courtney E. Wolfrum, Edward J. TI Rapid analysis of composition and reactivity in cellulosic biomass feedstocks with near-infrared spectroscopy SO BIOTECHNOLOGY FOR BIOFUELS LA English DT Article DE FT-NIR; NIR spectroscopy; Biomass conversion; Pretreatment; Enzymatic hydrolysis; High-throughput assay; Compositional analysis; Cellulosic biomass; Herbaceous feedstocks; PLS; Reactivity; Biofuels; Multivariate analysis ID PRETREATED CORN STOVER; CELL-WALL COMPOSITION; CHEMICAL-COMPOSITION; CALIBRATION MODELS; DIGESTIBILITY; SPECTROMETRY; HYDROLYSIS; MISCANTHUS; ETHANOL; SCALE AB Background: Obtaining accurate chemical composition and reactivity (measures of carbohydrate release and yield) information for biomass feedstocks in a timely manner is necessary for the commercialization of biofuels. Our objective was to use near-infrared (NIR) spectroscopy and partial least squares (PLS) multivariate analysis to develop calibration models to predict the feedstock composition and the release and yield of soluble carbohydrates generated by a bench-scale dilute acid pretreatment and enzymatic hydrolysis assay. Major feedstocks included in the calibration models are corn stover, sorghum, switchgrass, perennial cool season grasses, rice straw, and miscanthus. Results: We present individual model statistics to demonstrate model performance and validation samples to more accurately measure predictive quality of the models. The PLS-2 model for composition predicts glucan, xylan, lignin, and ash (wt%) with uncertainties similar to primary measurement methods. A PLS-2 model was developed to predict glucose and xylose release following pretreatment and enzymatic hydrolysis. An additional PLS-2 model was developed to predict glucan and xylan yield. PLS-1 models were developed to predict the sum of glucose/glucan and xylose/xylan for release and yield (grams per gram). The release and yield models have higher uncertainties than the primary methods used to develop the models. Conclusion: It is possible to build effective multispecies feedstock models for composition, as well as carbohydrate release and yield. The model for composition is useful for predicting glucan, xylan, lignin, and ash with good uncertainties. The release and yield models have higher uncertainties; however, these models are useful for rapidly screening sample populations to identify unusual samples. C1 [Payne, Courtney E.; Wolfrum, Edward J.] Natl Renewable Energy Lab, Natl Bioenergy Ctr, Golden, CO 80401 USA. RP Payne, CE (reprint author), Natl Renewable Energy Lab, Natl Bioenergy Ctr, 15013 Denver West Pkwy, Golden, CO 80401 USA. EM courtney.payne@nrel.gov OI Wolfrum, Edward/0000-0002-7361-8931 FU U.S. Department of Energy [DE-AC36-08GO28308]; National Renewable Energy Laboratory; USDOE Office of Energy Efficiency and Renewable Energy's BioEnergy Technologies Office FX The authors would like to acknowledge Amie Sluiter for her review of this manuscript, Stefanie Maletich for NIR scanning of all associated samples, and Ryan Ness and Darren Peterson for the reactivity work on which these models were based. The authors would also like to thank the Reviewers of this manuscript for their thoughtful and thorough review. This work was supported by the U.S. Department of Energy under Contract No. DE-AC36-08GO28308 with the National Renewable Energy Laboratory. Funding provided by USDOE Office of Energy Efficiency and Renewable Energy's BioEnergy Technologies Office. NR 40 TC 2 Z9 2 U1 3 U2 22 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1754-6834 J9 BIOTECHNOL BIOFUELS JI Biotechnol. Biofuels PD MAR 12 PY 2015 VL 8 AR 43 DI 10.1186/s13068-015-0222-2 PG 14 WC Biotechnology & Applied Microbiology; Energy & Fuels SC Biotechnology & Applied Microbiology; Energy & Fuels GA CE5UN UT WOS:000351901300001 PM 25834638 ER PT J AU Bai, Y He, HM Li, Y Li, ZR Zhou, ZJ Wang, JJ Wu, D Chen, W Gu, FL Sumpter, BG Huang, JS AF Bai, Yang He, Hui-Min Li, Ying Li, Zhi-Ru Zhou, Zhong-Jun Wang, Jia-Jun Wu, Di Chen, Wei Gu, Feng-Long Sumpter, Bobby G. Huang, Jingsong TI Electric Field Effects on the Intermolecular Interactions in Water Whiskers: Insight from Structures, Energetics, and Properties SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID CARBON NANOTUBES; POLYWATER; HYDROGEN; SPECTROSCOPY; INTERFACES; CHEMISTRY; GRADIENT; EMITTER; STORAGE; ENERGY AB Modulation of intermolecular interactions in response to external electric fields could be fundamental to the formation of unusual forms of water, such as water whiskers. However, a detailed understanding of the nature of intermolecular interactions in such systems is lacking. In this paper, we present novel theoretical results based on electron correlation calculations regarding the nature of H-bonds in water whiskers, which is revealed by studying their evolution under external electric fields with various field strengths. We find that the water whiskers consisting of 27 water molecules all have a chain-length dependent critical electric field. Under the critical electric field, the most compact chain structures are obtained, featuring very strong H-bonds, herein referred to as covalent H-bonds. In the case of a water dimer whisker, the bond length of the novel covalent H-bond shortens by 25%, the covalent bond order increases by 9 times, and accordingly the H-bond energy is strengthened by 5 times compared to the normal H-bond in a (H2O)(2) cluster. Below the critical electric field, it is observed that, with increasing field strength, H-bonding orbitals display gradual evolutions in the orbital energy, orbital ordering, and orbital nature (i.e., from typical p-style orbital to unusual s-style double H-bonding orbital). We also show that, beyond the critical electric field, a single water whisker may disintegrate to form a loosely bound zwitterionic chain due to a relay-style proton transfer, whereas two water whiskers may undergo intermolecular cross-linking to form a quasi-two-dimensional water network. Overall, these results help shed new insight on the effects of electric fields on water whisker formation. C1 [Bai, Yang; He, Hui-Min; Li, Ying; Li, Zhi-Ru; Zhou, Zhong-Jun; Wang, Jia-Jun; Wu, Di; Chen, Wei] Jilin Univ, State Key Lab Theoret & Computat Chem, Inst Theoret Chem, Changchun 130023, Peoples R China. [Gu, Feng-Long] S China Normal Univ, Ctr Computat Quantum Chem, Guangzhou 510631, Guangdong, Peoples R China. [Sumpter, Bobby G.; Huang, Jingsong] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Sumpter, Bobby G.; Huang, Jingsong] Oak Ridge Natl Lab, Div Math & Comp Sci, Oak Ridge, TN 37831 USA. RP Li, ZR (reprint author), Jilin Univ, State Key Lab Theoret & Computat Chem, Inst Theoret Chem, Changchun 130023, Peoples R China. EM lzr@jlu.edu.cn; gu@scnu.edu.cn; huangj3@ornl.gov RI Sumpter, Bobby/C-9459-2013; Huang, Jingsong/A-2789-2008; Wu, Di/Q-2590-2015 OI Sumpter, Bobby/0000-0001-6341-0355; Huang, Jingsong/0000-0001-8993-2506; FU National Natural Science Foundation of China [21173098, 21173095, 21103065, 21403083, 21043003]; Center for Nanophase Materials Sciences (CNMS) - Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX This work was financially supported by the National Natural Science Foundation of China (Nos. 21173098, 21173095, 21103065, 21403083, and 21043003) and by the Center for Nanophase Materials Sciences (CNMS), which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. Z.R.L. thanks Prof. Jia-Li Gao for the helpful discussions. NR 45 TC 5 Z9 5 U1 2 U2 43 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD MAR 12 PY 2015 VL 119 IS 10 BP 2083 EP 2090 DI 10.1021/jp511460c PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA CD6GZ UT WOS:000351188900028 PM 25695357 ER PT J AU Lee, CK Pao, CW Smit, B AF Lee, Cheng-Kuang Pao, Chun-Wei Smit, Berend TI PSII-LHCII Supercomplex Organizations in Photosynthetic Membrane by Coarse-Grained Simulation SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID TEMPERATURE-INDUCED INHIBITION; CYTOCHROME B(6)F COMPLEX; LIGHT-HARVESTING ANTENNA; PHOTOSYSTEM-II; THYLAKOID MEMBRANE; ARABIDOPSIS-THALIANA; CRYSTAL-STRUCTURE; SUPRAMOLECULAR ORGANIZATION; ANGSTROM RESOLUTION; PLANT CHLOROPLASTS AB Green plant Photosystem II (PSII) and light-harvesting complex II (LHCLI) in the stacked grana regions of thylakoid membranes can self-organize into various PSII LHCII supercomplexes With crystalline Of fluid-like supramolecular structures to adjust themselves with external stimuli suth as high/low light and 'temperatures, reuclering tunable solar light absorption spectrum and photosynthesis efficiencies. However, the mechanisms controlling the PSII LHCH Supercomplex organizations remain elusive: In this work, We constructed a coarse-grained (CO) model of the thylakoid membrane including lipid molecules and a PSII LHCII supercomplex considering association/dissociation of moderately bound-LHCHs. The CG interaction between CG beads were constructed based on electron microscope (EM) experimental results, and we were able to Simulate the PSII LHCII supramolecular organization of a 500 X 500 nm(2) thylakoid membrane, which is compatible with experiments. Our CGMD simulations can successfully reproduce order structures of PSII LHCII supercomplexes under various protein packing fractions, free-LHCII:PSII ratios, and temperatures, thereby providing insights into mechanisms leading to PSH LHCII stipercornplex organizations in photosynthetic membranes. C1 [Lee, Cheng-Kuang; Pao, Chun-Wei] Acad Sinica, Res Ctr Appl Sci, Taipei 11529, Taiwan. [Lee, Cheng-Kuang; Smit, Berend] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Smit, Berend] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Smit, Berend] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Smit, Berend] Ecole Polytech Fed Lausanne, ISIC, CH-1950 Sion, Switzerland. RP Pao, CW (reprint author), Acad Sinica, Res Ctr Appl Sci, Taipei 11529, Taiwan. EM cwpao@gate.sinica.edu.tw; Berend-Smit@berkeley.edu RI Pao, Chun-Wei/D-3307-2009; Smit, Berend/B-7580-2009; Lee, Cheng-Kuang/G-6390-2010 OI Pao, Chun-Wei/0000-0003-0821-7856; Smit, Berend/0000-0003-4653-8562; FU Academia Sinica of Taiwan R.O.C.; elite American universities and research institutes; National Science Council of Taiwan [99-2112-M-001-004-MY3, 102-2628-M-001-004-MY3]; Academia Sinica Thematic Project [AS-103-SS-A02]; FWP-SISGRKN from Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy FX C.-K.L. thanks S. Katira, Dr. A. Benjamini, Dr. A. R. Schneider, Prof. Y.-C. Cheng, and Prof. K. K. Niyogi for helpful discussions about the study and also thanks the support of the talent development program between Academia Sinica of Taiwan R.O.C. and elite American universities and research institutes; C.-W.P. thanks the National Science Council of Taiwan project No. 99-2112-M-001-004-MY3 and 102-2628-M-001-004-MY3, and Academia Sinica Thematic Project No. AS-103-SS-A02 for financial support, as well as computational support by the National Center of High-Performance Computing of Taiwan, ROC. This research was supported by Grant FWP-SISGRKN from the Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy. NR 52 TC 5 Z9 5 U1 4 U2 32 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAR 12 PY 2015 VL 119 IS 10 BP 3999 EP 4008 DI 10.1021/jp511277c PG 10 WC Chemistry, Physical SC Chemistry GA CD6GT UT WOS:000351188300013 PM 25679518 ER PT J AU Mildner, S Beleggia, M Mierwaldt, D Hansen, TW Wagner, JB Yazdi, S Kasama, T Ciston, J Zhu, YM Jooss, C AF Mildner, Stephanie Beleggia, Marco Mierwaldt, Daniel Hansen, Thomas W. Wagner, Jakob B. Yazdi, Sadegh Kasama, Takeshi Ciston, Jim Zhu, Yimei Jooss, Christian TI Environmental TEM Study of Electron Beam Induced Electrochemistry of Pr0.64Ca0.36MnO3 Catalysts for Oxygen Evolution SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID IN-SITU; MANGANITE PEROVSKITES; WATER OXIDATION; MICROSCOPY; OXIDES; INSULATORS; SCIENCE; EELS AB Environmental transmission electron microscopy (ETEVI) studies offer great potential for gathering atomic scale information on the electronic state of electrodes in contact with reactants. It also poses big challenges due to the impact of the high energy electron beam. In this article, we present an ETEM study of a Pr0.64Ca0.36MnO3 (PCMO) thin filth electrocatalySt for water splitting and Oxygen evolution in contact with water vapor: We show by means of off-axis electron holography and electrostatic modeling that the electron beam gives rise to a positive electric sample potential due to secondary electron emission. The value of the electric potential depends on the primary electron flux, the sample's electric Conductivity and grounding, and gas properties. We present evidence that two observed electrochemical reactions are driven by a beam induced electrostatic potential of the order of a volt. The first reaction is an anodic oxidation of oxygen depleted amorphous PCMO which results in recrystallization of the oxide. The Second reaction is oxygen evolution which can be detected by the oxidation of a silane additive and formation of SiO2-gamma at catalytically active surfaces. The quantification of beam induced potentials is an important step for future controlled electrochemical experiments in an ETEM. C1 [Mildner, Stephanie; Mierwaldt, Daniel; Jooss, Christian] Univ Gottingen, Inst Mat Phys, D-37077 Gottingen, Germany. [Beleggia, Marco; Hansen, Thomas W.; Wagner, Jakob B.; Yazdi, Sadegh; Kasama, Takeshi] Tech Univ Denmark, Ctr Electron Nanoscopy, DK-2800 Lyngby, Denmark. [Beleggia, Marco] Helmholtz Zentrum Berlin Mat & Energy, D-14109 Berlin, Germany. [Ciston, Jim] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Natl Ctr Electron Microscopy, Berkeley, CA 94720 USA. [Zhu, Yimei] Brookhaven Natl Lab, Dept Condensed Matter Phys & Mat Sci, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Jooss, C (reprint author), Univ Gottingen, Inst Mat Phys, Friedrich Hund Pl 1, D-37077 Gottingen, Germany. EM jooss@material.physik.uni-goettingen.de RI Wagner, Jakob/H-5392-2011; Foundry, Molecular/G-9968-2014; Kasama, Takeshi/K-5383-2012; Hansen, Thomas/H-5367-2011; OI Wagner, Jakob/0000-0002-2945-0190; Hansen, Thomas/0000-0002-1861-3054; Beleggia, Marco/0000-0002-2888-1888 FU DFG [SFB 1073] FX We thank the DFG for financial support within the SFB 1073, project C02. NR 41 TC 5 Z9 5 U1 6 U2 50 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAR 12 PY 2015 VL 119 IS 10 BP 5301 EP 5310 DI 10.1021/jp511628c PG 10 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CD6HB UT WOS:000351189100006 ER PT J AU Tafen, D Prezhdo, OV AF Tafen, De Nyago Prezhdo, Oleg V. TI Size and Temperature Dependence of Electron Transfer between CdSe Quantum Dots and a TiO2 Nanobelt SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID DOMAIN AB-INITIO; NONADIABATIC MOLECULAR-DYNAMICS; DYE-SENSITIZED TIO2; SOLAR-CELLS; SEMICONDUCTOR NANOCRYSTALS; CHARGE SEPARATION; PYXAID PROGRAM; INJECTION; NANOPARTICLES; RECOMBINATION AB Understanding charge transfer reactions between quantum dots (QD) and metal oxides is fundamental for improving photocatalytic, photovoltaic, and electronic devices. The complexity of these processes makes it difficult to find an optimum QD size with rapid charge injection and low recombination. We combine time-domain density functional theory with nonadiabatic molecular dynamics to investigate the size and temperature dependence of the experimentally studied electron transfer and charge recombination at CdSe QD-TiO2 nanobelt (NB) interfaces. The electron injection rate shows strong dependence on the QD size, increasing for small QDs. The rate exhibits Arrhenius temperature dependence, with the activation energy of the order of millielectronvolts. The charge recombination process occurs due to coupling of the electronic subsystem to vibrational modes of the TiO2 NB. Inelastic electron-phonon scattering happens on a picosecond time scale, with strong dependence on the QD size. Our simulations demonstrate that the electron-hole recombination rate decreases significantly as the QD size increases, in excellent agreement with experiments. The temperature dependence of the charge recombination rates can be successfully modeled within the framework of the Marcus theory through optimization of the electronic coupling and the reorganization energy. Our simulations indicate that by varying the QD size, one can modulate the photoinduced charge separation and charge recombination, fundamental aspects of the design principles for high-efficiency devices. C1 [Tafen, De Nyago] Natl Energy Technol Lab, Albany, OR 97321 USA. [Tafen, De Nyago] URS Corp, Albany, OR 97321 USA. [Prezhdo, Oleg V.] Univ So Calif, Dept Chem, Los Angeles, CA 90089 USA. RP Tafen, D (reprint author), Natl Energy Technol Lab, 1450 Queen Ave SW, Albany, OR 97321 USA. EM denyago.tafen@contr.netl.doe.gov; prezhdo@usc.edu OI Tafen, De Nyago/0000-0002-4360-9508 FU National Energy Technology Laboratory's ongoing research under the RES Contract [DE-FE0004000]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; US Department of Energy [DE-SC0006527]; Department of Energy, National Energy Technology Laboratory, an agency of the United States Government; URS Energy & Construction, Inc. FX The technical effort was performed in support of the National Energy Technology Laboratory's ongoing research under the RES Contract DE-FE0004000. Part of this research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract DE-AC02-05CH11231. D.N.T. thanks C. Matranga for fruitful discussions. O.V.P. acknowledges financial support of the US Department of Energy, Grant DE-SC0006527. This project was funded by the Department of Energy, National Energy Technology Laboratory, an agency of the United States Government, through a support contract with URS Energy & Construction, Inc. Neither the United States Government nor any agency thereof, nor any of their employees, nor URS Energy & Construction, Inc., nor any of their employees, makes any warranty, expressed or implied, or assumes any legal liability or responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would not infringe privately owned rights. Reference herein to any specific commercial product, process, or service by trade name, trademark, manufacturer, or otherwise, does not necessarily constitute or imply its endorsement, recommendation, or favoring by the United States Government or any agency thereof. The views and opinions of authors expressed herein do not necessarily state or reflect those of the United States Government or any agency thereof. NR 68 TC 8 Z9 8 U1 9 U2 89 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAR 12 PY 2015 VL 119 IS 10 BP 5639 EP 5647 DI 10.1021/jp5110278 PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA CD6HB UT WOS:000351189100045 ER PT J AU Li, L Parker, D Babkevich, P Yang, L Ronnow, HM Sefat, AS AF Li, L. Parker, D. Babkevich, P. Yang, L. Ronnow, H. M. Sefat, A. S. TI Superconductivity in semimetallic Bi3O2S3 SO PHYSICAL REVIEW B LA English DT Article ID THERMOELECTRIC PROPERTIES; BULK SUPERCONDUCTIVITY; BI4O4S3; SYSTEM AB Here we report a further investigation on the thermodynamic and transport properties, and an assessment of theoretical calculations, for the BiS2- layered Bi3O2S3 superconductor. The polycrystalline sample is synthesized with a superconducting transition temperature of T onset c = 5.75 K and T zero c = 4.03 K ( T mag c) that drops to 3.3 K by applying a hydrostatic pressure of 6 kbar. Density- of- states ( DOS) calculations give substantial hybridization between Bi, O, and S, with Bi the largest component of DOS, which supports the idea that the BiS2 layer is relevant for producing electron- phonon coupling. An analysis of previously published specific heat data for Bi3O2S3 is additionally suggestive of a strong electron- phonon interaction in the Bi- O- S system. The analysis of the Seebeck coefficient results strongly suggests that Bi3O2S3 is a semimetal. In fact, the semimetallic or narrow band gap behavior may occur in certain other materials in the BiS2- layered class of materials, such as Bi4O4S3. C1 [Li, L.; Parker, D.; Sefat, A. S.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Babkevich, P.; Yang, L.; Ronnow, H. M.] Ecole Polytech Fed Lausanne, LQM, CH-1015 Lausanne, Switzerland. [Yang, L.] Ecole Polytech Fed Lausanne, Lab Phys Complex Matter, CH-1015 Lausanne, Switzerland. RP Li, L (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RI EPFL, Physics/O-6514-2016; Sefat, Athena/R-5457-2016; OI Sefat, Athena/0000-0002-5596-3504; Li, Li/0000-0003-1683-8118 NR 21 TC 2 Z9 2 U1 4 U2 33 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAR 12 PY 2015 VL 91 IS 10 AR 104511 DI 10.1103/PhysRevB.91.104511 PG 5 WC Physics, Condensed Matter SC Physics GA CD8JG UT WOS:000351340500007 ER PT J AU Xu, B Dai, YM Shen, B Xiao, H Ye, ZR Forget, A Colson, D Feng, DL Wen, HH Homes, CC Qiu, XG Lobo, RPSM AF Xu, B. Dai, Y. M. Shen, B. Xiao, H. Ye, Z. R. Forget, A. Colson, D. Feng, D. L. Wen, H. H. Homes, C. C. Qiu, X. G. Lobo, R. P. S. M. TI Anomalous phonon redshift in K-doped BaFe2As2 iron pnictides SO PHYSICAL REVIEW B LA English DT Article AB The effect of K, Co, and P dopings on the lattice dynamics in the BaFe2As2 system is studied by infrared spectroscopy. We focus on the phonon at 253 cm- 1, the highest energy in- plane infrared- active Fe- As mode in BaFe2As2. Our studies show that Co and P dopings lead to a blueshift of this phonon in frequency, which can be simply interpreted by the change in lattice parameters induced by doping. In sharp contrast, an unusual redshift of the same mode was observed in the K- doped compound, at odds with the above explanation. This anomalous behavior in K- doped BaFe2As2 is more likely associated with the coupling between lattice vibrations and other channels, such as charge or spin. This coupling scenario is also supported by the asymmetric line shape and intensity growth of the phonon in the K- doped compound. C1 [Xu, B.; Lobo, R. P. S. M.] PSL Res Univ, ESPCI ParisTech, LPEM, F-75231 Paris 5, France. [Xu, B.; Shen, B.; Xiao, H.; Qiu, X. G.] Chinese Acad Sci, Beijing Natl Lab Condensed Matter Phys, Inst Phys, Beijing 100190, Peoples R China. [Dai, Y. M.; Homes, C. C.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Ye, Z. R.; Feng, D. L.] Fudan Univ, Dept Phys, State Key Lab Surface Phys, Shanghai 200433, Peoples R China. [Ye, Z. R.; Feng, D. L.] Fudan Univ, Adv Mat Lab, Shanghai 200433, Peoples R China. [Forget, A.; Colson, D.] CEA, SPEC, IRAMIS, F-91191 Gif Sur Yvette, France. [Wen, H. H.] Nanjing Univ, Natl Lab Solid State Microstruct, Nanjing 210093, Jiangsu, Peoples R China. [Wen, H. H.] Nanjing Univ, Dept Phys, Nanjing 210093, Jiangsu, Peoples R China. [Lobo, R. P. S. M.] CNRS, UMR 8213, F-75005 Paris, France. [Lobo, R. P. S. M.] Univ Paris 06, Sorbonne Univ, F-75005 Paris, France. RP Xu, B (reprint author), PSL Res Univ, ESPCI ParisTech, LPEM, 10 Rue Vauquelin, F-75231 Paris 5, France. EM ymdai@lanl.gov; lobo@espci.fr RI Dai, Yaomin/E-4259-2016; OI Dai, Yaomin/0000-0002-2464-3161; Lobo, Ricardo/0000-0003-2355-6856 NR 41 TC 6 Z9 6 U1 5 U2 23 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 12 PY 2015 VL 91 IS 10 AR 104510 DI 10.1103/PhysRevB.91.104510 PG 5 WC Physics, Condensed Matter SC Physics GA CD8JG UT WOS:000351340500006 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Eroe, J Friedl, M Fruehwirth, R Ghete, VM Hartl, C Hoermann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schofbeck, R Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Lauwers, J Luyckx, S Ochesanu, S Rougny, R Van De Klundert, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Daci, N Heracleous, N Keaveney, J Lowette, S Maes, M Olbrechts, A Python, Q Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Caillol, C Clerbaux, B De Lentdecker, G Dobur, D Favart, L Gay, APR Grebenyuk, 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Kaplan, S. Lath, A. Panwalkar, S. Park, M. Patel, R. Salur, S. Schnetzer, S. Sheffield, D. Somalwar, S. Stone, R. Thomas, S. Thomassen, P. Walker, M. Rose, K. Spanier, S. York, A. Bouhali, O. Castaneda Hernandez, A. Eusebi, R. Flanagan, W. Gilmore, J. Kamon, T. Khotilovich, V. Krutelyov, V. Montalvo, R. Osipenkov, I. Pakhotin, Y. Perloff, A. Roe, J. Rose, A. Safonov, A. Suarez, I. Tatarinov, A. Ulmer, K. A. Akchurin, N. Cowden, C. Damgov, J. Dragoiu, C. Dudero, P. R. Faulkner, J. Kovitanggoon, K. Kunori, S. Lee, S. W. Libeiro, T. Volobouev, I. Appelt, E. Delannoy, A. G. Greene, S. Gurrola, A. Johns, W. Maguire, C. Mao, Y. Melo, A. Sharma, M. Sheldon, P. Snook, B. Tuo, S. Velkovska, J. Arenton, M. W. Boutle, S. Cox, B. Francis, B. Goodell, J. Hirosky, R. Ledovskoy, A. Li, H. Lin, C. Neu, C. Wolfe, E. Wood, J. Clarke, C. Harr, R. Karchin, P. E. Don, C. Kottachchi Kankanamge Lamichhane, P. Sturdy, J. Belknap, D. A. Carlsmith, D. Cepeda, M. Dasu, S. Dodd, L. Duric, S. Friis, E. Hall-Wilton, R. Herndon, M. Herve, A. Klabbers, P. Lanaro, A. Lazaridis, C. Levine, A. Loveless, R. Mohapatra, A. Ojalvo, I. Perry, T. Pierro, G. A. Polese, G. Ross, I. Sarangi, T. Savin, A. Smith, W. H. Taylor, D. Vuosalo, C. Woods, N. CA CMS Collaboration TI Search for resonances and quantum black holes using dijet mass spectra in proton-proton collisions at root s=8 TeV SO PHYSICAL REVIEW D LA English DT Article ID HADRON COLLIDERS; PHYSICS; PHENOMENOLOGY; HIERARCHY AB A search for resonances and quantum black holes is performed using the dijet mass spectra measured in proton-proton collisions at root s = 8 TeV with the CMS detector at the LHC. The data set corresponds to an integrated luminosity of 19.7 fb(-1). In a search for narrow resonances that couple to quark-quark, quark-gluon, or gluon-gluon pairs, model-independent upper limits, at 95% confidence level, are obtained on the production cross section of resonances, with masses above 1.2 TeV. When interpreted in the context of specific models the limits exclude string resonances with masses below 5.0 TeV; excited quarks below 3.5 TeV; scalar diquarks below 4.7 TeV; W' bosons below 1.9 TeV or between 2.0 and 2.2 TeV; Z' bosons below 1.7 TeV; and Randall-Sundrum gravitons below 1.6 TeV. A separate search is conducted for narrow resonances that decay to final states including b quarks. The first exclusion limit is set for excited b quarks, with a lower mass limit between 1.2 and 1.6 TeV depending on their decay properties. Searches are also carried out for wide resonances, assuming for the first time width-to-mass ratios up to 30%, and for quantum black holes with a range of model parameters. The wide resonance search excludes axigluons and colorons with mass below 3.6 TeV, and color-octet scalars with mass below 2.5 TeV. Lower bounds between 5.0 and 6.3 TeV are set on the masses of quantum black holes. C1 [Khachatryan, V.; Sirunyan, A. 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O.; Salfeld-Nebgen, J.; Saxena, P.; Schoerner-Sadenius, T.; Schroeder, M.; Seitz, C.; Spannagel, S.; Trevino, A. D. R. Vargas; Walsh, R.; Wissing, C.] Deutsch Elekt Synchrotron, Hamburg, Germany. [Blobel, V.; Vignali, M. Centis; Draeger, A. R.; Erfle, J.; Garutti, E.; Goebel, K.; Goerner, M.; Haller, J.; Hoffmann, M.; Hoeing, R. S.; Junkes, A.; Kirschenmann, H.; Klanner, R.; Kogler, R.; Lapsien, T.; Lenz, T.; Marchesini, I.; Marconi, D.; Ott, J.; Peiffer, T.; Perieanu, A.; Pietsch, N.; Poehlsen, J.; Poehlsen, T.; Rathjens, D.; Sander, C.; Schettler, H.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Seidel, M.; Sola, V.; Stadie, H.; Steinbruck, G.; Troendle, D.; Usai, E.; Vanelderen, L.; Vanhoefer, A.] Univ Hamburg, Hamburg, Germany. [Barth, C.; Baus, C.; Berger, J.; Boeser, C.; Butz, E.; Chwalek, T.; De Boer, W.; Descroix, A.; Dierlamm, A.; Feindt, M.; Frensch, F.; Giffels, M.; Gilbert, A.; Hartmann, F.; Hauth, T.; Husemann, U.; Kornmayer, A.; Pardo, P. Lobelle; Mozer, M. U.; Mueller, T.; Mueller, Th.; Nuernberg, A.; Quast, G.; Rabbertz, K.; Roecker, S.; Simonis, H. J.; Stober, F. M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weiler, T.; Wolf, R.] Univ Karlsruhe, Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Giakoumopoulou, V. A.; Kyriakis, A.; Loukas, D.; Markou, A.; Markou, C.; Psallidas, A.; Topsis-Giotis, I.] NCSR Demokritos, INPP, Aghia Paraskevi, Greece. [Agapitos, A.; Kesisoglou, S.; Panagiotou, A.; Saoulidou, N.; Stiliaris, E.; Tziaferi, E.] Univ Athens, Athens, Greece. [Aslanoglou, X.; Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Manthos, N.; Papadopoulos, I.; Paradas, E.; Strologas, J.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.] Wigner Res Ctr Phys, Budapest, Hungary. [Beni, N.; Czellar, S.; Karancsi, J.; Molnar, J.; Palinkas, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Makovec, A.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, H-4012 Debrecen, Hungary. [Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Beri, S. B.; Bhatnagar, V.; Gupta, R.; Bhawandeep, U.; Kalsi, A. K.; Kaur, M.; Kumar, R.; Mittal, M.; Nishu, N.; Singh, J. B.] Panjab Univ, Chandigarh 160014, India. [Kumar, Ashok; Kumar, Arun; Ahuja, S.; Bhardwaj, A.; Choudhary, B. C.; Kumar, A.; Malhotra, S.; Naimuddin, M.; Ranjan, K.; Sharma, V.] Univ Delhi, Delhi 110007, India. [Banerjee, S.; Bhattacharya, S.; Chatterjee, K.; Dutta, S.; Gomber, B.; Jain, Sa.; Jain, Sh.; Khurana, R.; Modak, A.; Mukherjee, S.; Roy, D.; Sarkar, S.; Sharan, M.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Dutta, D.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Mumbai 400085, Maharashtra, India. [Aziz, T.; Banerjee, S.; Bhowmik, S.; Chatterjee, R. M.; Dewanjee, R. K.; Dugad, S.; Ganguly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Kole, G.; Kumar, S.; Maity, M.; Majumder, G.; Mazumdar, K.; Mohanty, G. B.; Parida, B.; Sudhakar, K.; Wickramage, N.; Penzo, A.] Tata Inst Fundamental Res, Mumbai 400005, Maharashtra, India. [Sharma, S.] Indian Inst Sci Educ & Res IISER, Pune, Maharashtra, India. [Bakhshiansohi, H.; Behnamian, H.; Etesami, S. M.; Fahim, A.; Goldouzian, R.; Khakzad, M.; Najafabadi, M. Mohammadi; Naseri, M.; Mehdiabadi, S. Paktinat; Hosseinabadi, F. Rezaei; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Felcini, M.; Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Abbrescia, M.; Calabria, C.; Chhibra, S. S.; Colaleo, A.; Creanza, D.; Cristella, L.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; My, S.; Nuzzo, S.; Pompili, A.; Pugliese, G.; Radogna, R.; Selvaggi, G.; Sharma, A.; Silvestris, L.; Venditti, R.; Verwilligen, P.] INFN Sez Bari, Bari, Italy. [Abbrescia, M.; Calabria, C.; Chhibra, S. S.; Cristella, L.; De Palma, M.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Montanari, A.; Navarria, F. L.; Perrotta, A.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] INFN Sez Bologna, Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Cavallo, F. R.; Codispoti, G.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Navarria, F. L.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] INFN Sez Catania, Catania, Italy. [Albergo, S.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Giordano, F.] CSFNSM, Catania, Italy. [Barbagli, G.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gallo, E.; Gonzi, S.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] INFN Sez Firenze, Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Tropiano, A.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Fabbri, F.; Piccolo, D.] INFN Lab Nazl Frascati, Frascati, Italy. [Ferretti, R.; Lo Vetere, M.; Robutti, E.; Tosi, S.; Dinardo, M. E.] INFN Sez Genova, Genoa, Italy. [Ferretti, R.; Robutti, E.; Dinardo, M. E.] Univ Genoa, Genoa, Italy. [Fiorendi, S.; Gennai, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] INFN Sez Milano Bicocca, Milan, Italy. [Fiorendi, S.; Gennai, S.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Manzoni, R. A.; Martelli, A.; Marzocchi, B.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Di Guida, S.; Fabozzi, F.; Iorio, A. O. M.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.] INFN Sez Napoli, Naples, Italy. [Iorio, A. O. M.] Univ Naples Federico II, Naples, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata Potenza, Naples, Italy. [Di Guida, S.; Meola, S.] Univ G Marconi Roma, Naples, Italy. [Azzi, P.; Bacchetta, N.; Bellato, M.; Bisello, D.; Carlin, R.; Checchia, P.; Dall'Osso, M.; Dorigo, T.; Fantinel, S.; Gasparini, F.; Gasparini, U.; Gonella, F.; Gozzelino, A.; Lacaprara, S.; Margoni, M.; Meneguzzo, A. T.; Montecassiano, F.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Zotto, P.; Zucchetta, A.] INFN Sez Padova, Padua, Italy. [Bisello, D.; Carlin, R.; Dall'Osso, M.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.] Univ Padua, Padua, Italy. Univ Trento Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vitulo, P.] INFN Sez Pavia, Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Saha, A.; Santocchia, A.; Spiezia, A.] INFN Sez Perugia, Perugia, Italy. [Biasini, M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Santocchia, A.; Spiezia, A.] Univ Perugia, Perugia, Italy. [Aleksandrov, A.; Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Fedi, G.; Fiori, F.; Foa, L.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Moon, C. S.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] INFN Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Serban, A. T.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; Ligabue, F.; Vernieri, C.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; D'imperio, G.; Del Re, D.; Diemoz, M.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Soffi, L.; Traczyk, P.] INFN Sez Roma, Rome, Italy. [Barone, L.; D'imperio, G.; Del Re, D.; Longo, E.; Margaroli, F.; Micheli, F.; Organtini, G.; Rahatlou, S.; Santanastasio, F.; Soffi, L.; Traczyk, P.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Covarelli, R.; Degano, A.; Demaria, N.; Finco, L.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] INFN Sez Torino, Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Casasso, S.; Costa, M.; Degano, A.; Finco, L.; Migliore, E.; Monaco, V.; Pacher, L.; Angioni, G. L. Pinna; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Schizzi, A.; Umer, T.; Zanetti, A.] INFN Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Schizzi, A.; Umer, T.] Univ Trieste, Trieste, Italy. [Chang, S.; Kropivnitskaya, A.] Kangwon Natl Univ, Chunchon, South Korea. [Nam, S. K.; Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Park, H.; Sakharov, A.; Son, D. C.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, T. J.; Ryu, M. S.] Chonbuk Natl Univ, Jeonju 561756, South Korea. [Kim, J. Y.; Moon, D. H.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, Y.; Lee, B.; Lee, K. S.; Park, S. K.; Roh, Y.; Yoo, H. D.] Korea Univ, Seoul, South Korea. Seoul Natl Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, I. C.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, D.; Kwon, E.; Lee, J.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.] Vilnius State Univ, Vilnius, Lithuania. [Komaragiri, J. R.; Ali, M. A. B. Md] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Linares, E. Casimiro; Castilla-Valdez, H.; De la Cruz-Burelo, E.; la Cruz, I. Heredia-De; Hernandez-Almada, A.; Lopez-Fernandez, R.; Sanchez-Hernandez, A.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Moreno, S. Carrillo; Valencia, F. Vazquez] Univ Iberoamer, Mexico City, DF, Mexico. [Pedraza, I.; Ibarguen, H. A. Salazar] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Pineda, A. Morelos] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Reucroft, S.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, A.; Ahmad, M.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bargassa, P.; Da Cruz E Silva, C. Beirao; Faccioli, P.; Parracho, P. G. Ferreira; Gallinaro, M.; Iglesias, L. Lloret; Nguyen, F.; Antunes, J. Rodrigues; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Kuznetsova, E.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Pozdnyakov, I.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia. [Adzic, P.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.] Univ Belgrade, Fac Phys & Vinca Inst Nucl Sci, Belgrade, Serbia. [Maestre, J. Alcaraz; Battilana, C.; Calvo, E.; Cerrada, M.; Llatas, M. Chamizo; Colino, N.; De la Cruz, B.; Peris, A. Delgado; Dominguez Vazquez, D.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.] CIEMAT, Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Graziano, A.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.; Penzo, A.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Aleksandrov, A.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; David, A.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dorney, B.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Franzoni, G.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Hansen, M.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Loureno, C.; Magini, N.; Malgeri, L.; Mannelli, M.; Marrouche, J.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Orsini, L.; Pape, L.; Perez, E.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Pimi, M.; Piparo, D.; Plagge, M.; Racz, A.; Rolandi, G.; Rovere, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Sharma, A.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Steggemann, J.; Stieger, B.; Stoye, M.; Takahashi, Y.; Treille, D.; Tsirou, A.; Veres, G. I.; Wardle, N.; Woehri, H. K.; Wollny, H.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Buchmann, M. A.; Casal, B.; Chanon, N.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eller, P.; Grab, C.; Hits, D.; Hoss, J.; Lustermann, W.; Mangano, B.; Marini, A. C.; Marionneau, M.; Martinez Ruiz del Arbol, P.; Masciovecchio, M.; Meister, D.; Mohr, N.; Musella, P.; Naegeli, C.; Nessi-Tedaldi, F.; Pandolfi, F.; Pauss, F.; Perrozzi, L.; Peruzzi, M.; Quittnat, M.; Rebane, L.; Rossini, M.; Starodumov, A.; Takahashi, M.; Theofilatos, K.; Wallny, R.; Weber, H. A.] ETH, Inst Particle Phys, Zurich, Switzerland. [Amsler, C.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Ngadiuba, J.; Pinna, D.; Robmann, P.; Ronga, F. J.; Taroni, S.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli, Taiwan. [Chang, P.; Chang, Y. H.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Grundler, U.; Hou, W. -S.; Liu, Y. F.; Lu, R. -S.; Moya, M. Minanno; Petrakou, E.; Tzeng, Y. M.; Wilken, R.] Natl Taiwan Univ NTU, Taipei, Taiwan. [Asavapibhop, B.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Fac Sci, Dept Phys, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Gamsizkan, H.; Isildak, B.; Karapinar, G.; Ocalan, K.; Sekmen, S.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Albayrak, E. A.; Gulmez, E.; Kaya, M.; Kaya, O.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cankocak, K.; Vardarli, F. I.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Flacher, H.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Sakuma, T.; El Nasr-Storey, S. Seif; Senkin, S.; Smith, V. J.] Univ Bristol, Bristol, Avon, England. [Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Williams, T.; Womersley, W. J.; Worm, S. D.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Dauncey, P.; Davies, G.; Della Negra, M.; Dunne, P.; Elwood, A.; Ferguson, W.; Fulcher, J.; Futyan, D.; Hall, G.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Mathias, B.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Pastika, N.; Scarborough, T.; Wu, Z.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Lawson, P.; Richardson, C.; Rohlf, J.; John, J. St.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Berry, E.; Bhattacharya, S.; Christopher, G.; Cutts, D.; Demiragli, Z.; Dhingra, N.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.; Swanson, J.] Brown Univ, Providence, RI USA. [Breedon, R.; Breto, G.; De La Barca Sanchez, M. Calderon; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Lander, R.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Cousins, R.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Rakness, G.; Takasugi, E.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Rikova, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Negrete, M. Olmedo; Shrinivas, A.; Sumowidagdo, S.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Holzner, A.; Kelley, R.; Klein, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Palmer, C.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Tadel, M.; Tu, Y.; Vartak, A.; Welke, C.; Wuerthwein, F.; Yagil, A.; Della Porta, G. Zevi] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bradmiller-Feld, J.; Campagnari, C.; Danielson, T.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Incandela, J.; Justus, C.; Mccoll, N.; Mullin, S. D.; Richman, J.; Stuart, D.; To, W.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Pierini, M.; Spiropulu, M.; Vlimant, J. R.; Wilkinson, R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Iiyama, Y.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Krohn, M.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Skinnari, L.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.; Winn, D.] Cornell Univ, Ithaca, NY USA. [Abdullin, S.] Fairfield Univ, Fairfield, CT 06430 USA. [Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Klima, B.; Kreis, B.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mishra, K.; Mrenna, S.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Sexton-Kennedy, E.; Soha, A.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitbeck, A.; Whitmore, J.; Yang, F.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Carver, M.; Curry, D.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Field, R. D.; Fisher, M.; Furic, I. K.; Hugon, J.; Konigsberg, J.; Korytov, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Rinkevicius, A.; Shchutska, L.; Snowball, M.; Sperka, D.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, J. R.; Adams, T.; Askew, A.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Kurt, P.; O'Brien, C.; Gonzalez, I. D. Sandoval; Silkworth, C.; Turner, P.; Varelas, N.] UIC, Chicago, IL USA. [Bilki, B.; Clarida, W.; Dilsiz, K.; Haytmyradov, M.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Rahmat, R.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Anderson, I.; Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Swartz, M.; Xiao, M.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Bruner, C.; Gray, J.; Kenny, R. P., III; Majumder, D.; Malek, M.; Murray, M.; Noonan, D.; Sanders, S.; Sekaric, J.; Stringer, R.; Wang, Q.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Chakaberia, I.; Ivanov, A.; Kaadze, K.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Skhirtladze, N.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Belloni, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Jabeen, S.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Mignerey, A. C.; Pedro, K.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Bierwagen, K.; Busza, W.; Cali, I. A.; Di Matteo, L.; Gomez Ceballos, G.; Goncharov, M.; Gulhan, D.; Klute, M.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Sumorok, K.; Velicanu, D.; Veverka, J.; Wyslouch, B.; Yang, M.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; Gude, A.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Nourbakhsh, S.; Rusack, R.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Gonzalez Suarez, R.; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Meier, F.; Ratnikov, F.; Snow, G. R.; Zvada, M.] Univ Nebraska, Lincoln, NE USA. [Dolen, J.; Godshalk, A.; Iashvili, I.; Kharchilava, A.; Kumar, A.; Rappoccio, S.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; Trocino, D.; Wang, R. -J.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Hahn, K. A.; Kubik, A.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Brinkerhoff, A.; Chan, K. M.; Drozdetskiy, A.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Lynch, S.; Marinelli, N.; Musienko, Y.; Pearson, T.; Planer, M.; Ruchti, R.; Smith, G.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hart, A.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Luo, W.; Puigh, D.; Rodenburg, M.; Winer, B. L.; Wolfe, H.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Driga, O.; Elmer, P.; Hardenbrook, J.; Hebda, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Brownson, E.; Malik, S.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA. [Barnes, V. E.; Benedetti, D.; Bortoletto, D.; De Mattia, M.; Gutay, L.; Hu, Z.; Jha, M. K.; Jones, M.; Kress, M.; Leonardo, N.; Miller, D. H.; Neumeister, N.; Primavera, F.; Radburn-Smith, B. C.; Shi, X.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.; Zablocki, J.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.; Stupak, J.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Ecklund, K. M.; Geurts, F. J. M.; Li, W.; Michlin, B.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; De Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Galanti, M.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Hindrichs, O.; Khukhunaishvili, A.; Korjenevski, S.; Petrillo, G.; Verzetti, M.; Vishnevskiy, D.] Univ Rochester, Rochester, NY 14627 USA. [Ciesielski, R.; Demortier, L.; Goulianos, K.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Kaplan, S.; Lath, A.; Panwalkar, S.; Park, M.; Patel, R.; Salur, S.; Schnetzer, S.; Sheffield, D.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Rose, K.; Spanier, S.; York, A.] Univ Tennessee, Knoxville, TN USA. [Bouhali, O.; Castaneda Hernandez, A.; Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Khotilovich, V.; Krutelyov, V.; Montalvo, R.; Osipenkov, I.; Pakhotin, Y.; Perloff, A.; Roe, J.; Rose, A.; Safonov, A.; Suarez, I.; Tatarinov, A.; Ulmer, K. A.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kovitanggoon, K.; Kunori, S.; Lee, S. W.; Libeiro, T.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Johns, W.; Maguire, C.; Mao, Y.; Melo, A.; Sharma, M.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN 37235 USA. [Arenton, M. W.; Boutle, S.; Cox, B.; Francis, B.; Hirosky, R.; Ledovskoy, A.; Li, H.; Lin, C.; Neu, C.; Wolfe, E.; Wood, J.; Clarke, C.] Univ Virginia, Charlottesville, VA USA. [Goodell, J.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sturdy, J.] Wayne State Univ, Detroit, MI USA. [Belknap, D. A.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Dodd, L.; Duric, S.; Friis, E.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Lanaro, A.; Lazaridis, C.; Levine, A.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ross, I.; Sarangi, T.; Savin, A.; Smith, W. H.; Taylor, D.; Vuosalo, C.; Woods, N.] Univ Wisconsin, Madison, WI 53706 USA. [Fruehwirth, R.; Jeitler, M.; Krammer, M.; Wulz, C. -E.] Vienna Univ Technol, A-1040 Vienna, Austria. [Rabady, D.; Pernie, L.; Genchev, V.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Beluffi, C.] Univ Haute Alsace Mulhouse, CNRS IN2P3, Univ Strasbourg, Inst Pluridisciplinaire Hubert Curien, Strasbourg, France. [Giammanco, A.] NICPB, Tallinn, Estonia. [Popov, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Chinellato, J.; Tonelli Manganote, E. J.] Univ Estadual Campinas, Campinas, Brazil. [Plestina, R.] Ecole Polytech, IN2P3 CNRS, Lab Leprince Ringuet, Palaiseau, France. [Finger, M., Jr.] Joint Inst Nucl Res, Dubna, Russia. [Assran, Y.] Suez Univ, Suez, Egypt. [Elgammal, S.] British Univ Egypt, Cairo, Egypt. [Kamel, A. Ellithi] Cairo Univ, Cairo, Egypt. [Radi, A.] Ain Shams Univ, Cairo, Egypt. [Radi, A.] Sultan Qaboos Univ, Muscat, Oman. [Agram, J. -L.; Conte, E.; Fontaine, J. -C.] Univ Haute Alsace, Mulhouse, France. [Bagaturia, I.] Ilia State Univ, Tbilisi, Rep of Georgia. [Hempel, M.; Karacheban, O.; Lohmann, W.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Horvath, D.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Vesztergombi, G.; Veres, G. I.] Eotvos Lorand Univ, Budapest, Hungary. [Karancsi, J.] Univ Debrecen, H-4012 Debrecen, Hungary. [Bhowmik, S.; Maity, M.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Gurtu, A.] King Abdulaziz Univ, Jeddah 21413, Saudi Arabia. [Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka. [Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Fahim, A.] Univ Tehran, Dept Engn Sci, Tehran, Iran. [Safarzadeh, B.] Islamic Azad Univ, Sci & Res Branch, Plasma Phys Res Ctr, Tehran, Iran. [Androsov, K.; Ciocci, M. A.; Grippo, M. T.; Squillacioti, P.] Univ Siena, I-53100 Siena, Italy. [Moon, C. S.] CNRS, IN2P3, Paris, France. [Savoy-Navarro, A.] Purdue Univ, W Lafayette, IN 47907 USA. [Matveev, V.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Kim, V.] St Petersburg State Polytech Univ, St Petersburg, Russia. [Dubinin, M.] CALTECH, Pasadena, CA 91125 USA. [Adzic, P.] Univ Belgrade, Fac Phys, New Delhi 11001, India. [Colafranceschi, S.] Univ Rome, Fac Ingn, Rome, Italy. [Rolandi, G.] Ist Nazl Fis Nucl, Scuola Normale & Sez, Pisa, Italy. [Sphicas, P.] Univ Athens, Athens, Greece. [Naegeli, C.] Paul Scherrer Inst, Villigen, Switzerland. [Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Bakirci, M. N.; Ozturk, S.; Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey. [Cerci, S.; Cerci, D. Sunar; Tali, B.] Adiyaman Univ, Adiyaman, Turkey. [Kangal, E. E.] Mersin Univ, Mersin, Turkey. [Onengut, G.] Cag Univ, Mersin, Turkey. [Ozdemir, K.] Piri Reis Univ, Istanbul, Turkey. [Gamsizkan, H.] Anadolu Univ, Eskisehir, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Ocalan, K.] Necmettin Erbakan Univ, Konya, Turkey. [Ocalan, K.] Necmettin Erbakan Univ, Konya, Turkey. [Albayrak, E. A.; Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Kaya, M.] Marmara Univ, Istanbul, Turkey. [Kaya, O.] Kafkas Univ, Kars, Turkey. [Yetkin, T.] Yildiz Tekn Univ, Istanbul, Turkey. [Newbold, D. M.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Bilki, B.] Argonne Natl Lab, Argonne, IL 60439 USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Bouhali, O.] Texas A&M Univ Qatar, Doha, Qatar. [Kamon, T.] Kyungpook Natl Univ, Daegu, South Korea. RP Khachatryan, V (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Hernandez Calama, Jose Maria/H-9127-2015; ciocci, maria agnese /I-2153-2015; Bedoya, Cristina/K-8066-2014; My, Salvatore/I-5160-2015; Benussi, Luigi/O-9684-2014; Lo Vetere, Maurizio/J-5049-2012; Ragazzi, Stefano/D-2463-2009; Grandi, Claudio/B-5654-2015; Rovelli, Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Dogra, Sunil /B-5330-2013; Petrushanko, Sergey/D-6880-2012; Wulz, Claudia-Elisabeth/H-5657-2011; Belyaev, Alexander/F-6637-2015; Manganote, Edmilson/K-8251-2013; Stahl, Achim/E-8846-2011; Trocsanyi, Zoltan/A-5598-2009; Cavallo, Nicola/F-8913-2012; Lokhtin, Igor/D-7004-2012; Bernardes, Cesar Augusto/D-2408-2015; VARDARLI, Fuat Ilkehan/B-6360-2013; Sen, Sercan/C-6473-2014; D'Alessandro, Raffaello/F-5897-2015; Montanari, Alessandro/J-2420-2012; Menasce, Dario Livio/A-2168-2016; Rolandi, Luigi (Gigi)/E-8563-2013; Sguazzoni, Giacomo/J-4620-2015; Ligabue, Franco/F-3432-2014; Goh, Junghwan/Q-3720-2016; Ruiz, Alberto/E-4473-2011; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Paulini, Manfred/N-7794-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Ogul, Hasan/S-7951-2016; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Da Silveira, Gustavo Gil/N-7279-2014; Mora Herrera, Maria Clemencia/L-3893-2016; Mundim, Luiz/A-1291-2012; Haj Ahmad, Wael/E-6738-2016; Konecki, Marcin/G-4164-2015; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Calderon, Alicia/K-3658-2014; Cerrada, Marcos/J-6934-2014; Perez-Calero Yzquierdo, Antonio/F-2235-2013; Novaes, Sergio/D-3532-2012; Della Ricca, Giuseppe/B-6826-2013; Chinellato, Jose Augusto/I-7972-2012; Tomei, Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Tinoco Mendes, Andre David/D-4314-2011; Seixas, Joao/F-5441-2013; Leonidov, Andrey/M-4440-2013; Andreev, Vladimir/M-8665-2015; Cakir, Altan/P-1024-2015; Matorras, Francisco/I-4983-2015; Gennai, Simone/P-2880-2015; TUVE', Cristina/P-3933-2015; Dudko, Lev/D-7127-2012; KIM, Tae Jeong/P-7848-2015; Paganoni, Marco/A-4235-2016; Azarkin, Maxim/N-2578-2015; de Jesus Damiao, Dilson/G-6218-2012; Calvo Alamillo, Enrique/L-1203-2014; Flix, Josep/G-5414-2012 OI Hernandez Calama, Jose Maria/0000-0001-6436-7547; ciocci, maria agnese /0000-0003-0002-5462; Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680; Benussi, Luigi/0000-0002-2363-8889; Lo Vetere, Maurizio/0000-0002-6520-4480; Ragazzi, Stefano/0000-0001-8219-2074; Grandi, Claudio/0000-0001-5998-3070; Rovelli, Tiziano/0000-0002-9746-4842; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Belyaev, Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Montanari, Alessandro/0000-0003-2748-6373; Ciulli, Vitaliano/0000-0003-1947-3396; Androsov, Konstantin/0000-0003-2694-6542; Fiorendi, Sara/0000-0003-3273-9419; Martelli, Arabella/0000-0003-3530-2255; Gonzi, Sandro/0000-0003-4754-645X; Levchenko, Petr/0000-0003-4913-0538; Heath, Helen/0000-0001-6576-9740; Gallinaro, Michele/0000-0003-1261-2277; Menasce, Dario Livio/0000-0002-9918-1686; Gerosa, Raffaele/0000-0001-8359-3734; Bilki, Burak/0000-0001-9515-3306; Rolandi, Luigi (Gigi)/0000-0002-0635-274X; Sguazzoni, Giacomo/0000-0002-0791-3350; Casarsa, Massimo/0000-0002-1353-8964; Ligabue, Franco/0000-0002-1549-7107; Diemoz, Marcella/0000-0002-3810-8530; Tricomi, Alessia Rita/0000-0002-5071-5501; Ghezzi, Alessio/0000-0002-8184-7953; Demaria, Natale/0000-0003-0743-9465; Benaglia, Andrea Davide/0000-0003-1124-8450; Covarelli, Roberto/0000-0003-1216-5235; Goh, Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787; Ogul, Hasan/0000-0002-5121-2893; Longo, Egidio/0000-0001-6238-6787; Di Matteo, Leonardo/0000-0001-6698-1735; Baarmand, Marc/0000-0002-9792-8619; Boccali, Tommaso/0000-0002-9930-9299; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Mundim, Luiz/0000-0001-9964-7805; Haj Ahmad, Wael/0000-0003-1491-0446; Konecki, Marcin/0000-0001-9482-4841; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Cerrada, Marcos/0000-0003-0112-1691; Perez-Calero Yzquierdo, Antonio/0000-0003-3036-7965; Novaes, Sergio/0000-0003-0471-8549; Della Ricca, Giuseppe/0000-0003-2831-6982; Chinellato, Jose Augusto/0000-0002-3240-6270; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Seixas, Joao/0000-0002-7531-0842; Matorras, Francisco/0000-0003-4295-5668; TUVE', Cristina/0000-0003-0739-3153; Dudko, Lev/0000-0002-4462-3192; KIM, Tae Jeong/0000-0001-8336-2434; Paganoni, Marco/0000-0003-2461-275X; de Jesus Damiao, Dilson/0000-0002-3769-1680; Calvo Alamillo, Enrique/0000-0002-1100-2963; Flix, Josep/0000-0003-2688-8047 FU Science and Technology Facilities Council [CMS, ST/K001604/1] NR 61 TC 70 Z9 70 U1 15 U2 72 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD MAR 12 PY 2015 VL 91 IS 5 AR 052009 DI 10.1103/PhysRevD.91.052009 PG 29 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CD8KD UT WOS:000351342800001 ER PT J AU Mirbabayi, M Senatore, L Silverstein, E Zaldarriaga, M AF Mirbabayi, Mehrdad Senatore, Leonardo Silverstein, Eva Zaldarriaga, Matias TI Gravitational waves and the scale of inflation SO PHYSICAL REVIEW D LA English DT Article ID POLARIZATION AB We revisit alternative mechanisms of gravitational wave production during inflation and argue that they generically emit a non-negligible amount of scalar fluctuations. We find the scalar power is larger than the tensor power by a factor of order 1/epsilon(2). For an appreciable tensor contribution, the associated scalar emission completely dominates the zero-point fluctuations of the inflaton, resulting in a tensor-to-scalar ratio r similar to epsilon(2). A more quantitative result can be obtained if one further assumes that gravitational waves are emitted by localized subhorizon processes, giving r(max) similar or equal to 0.3 epsilon(2). However, epsilon is generally time dependent, and this result for r depends on its instantaneous value during the production of the sources, rather than just its average value, somewhat relaxing constraints from the tilt n(s). We calculate the scalar 3-point correlation function in the same class of models and show that non-Gaussianity cannot be made arbitrarily small, i.e. f(NL) >= 1, independently of the value of r. Possible exceptions in multifield scenarios are discussed. C1 [Mirbabayi, Mehrdad; Zaldarriaga, Matias] Inst Adv Study, Princeton, NJ 08540 USA. [Senatore, Leonardo; Silverstein, Eva] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Senatore, Leonardo; Silverstein, Eva] Stanford Univ, SLAC, Stanford, CA 94305 USA. RP Mirbabayi, M (reprint author), Inst Adv Study, Olden Lane, Princeton, NJ 08540 USA. FU National Science Foundation [PHY-1314311, PHY-0855425, PHY-1068380, PHY-0756174, PHY11-25915, AST-0907969, PHY-1213563, AST-1409709]; Department of Energy Early Career Award [DE-FG02-12ER41854]; Department of Energy [DE-AC03-76SF00515] FX We thank S. Adler, G. D'Amico, R. Flauger, A. Gruzinov, M. Kleban, S. Mukohyama, R. Namba, M. Peloso, and G. Shiu for stimulating discussions. M. M. is supported by National Science Foundation Grants No. PHY-1314311 and No. PHY-0855425. L. S. is supported by Department of Energy Early Career Award No. DE-FG02-12ER41854 and the National Science Foundation Grant No. PHY-1068380. E. S. is supported in part by the National Science Foundation under Grants No. PHY-0756174 and No. PHY11-25915 and by the Department of Energy under Contract No. DE-AC03-76SF00515. M. Z. is supported in part by the National Science Foundation Grants No. AST-0907969, No. PHY-1213563 and No. AST-1409709. NR 32 TC 14 Z9 14 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD MAR 12 PY 2015 VL 91 IS 6 AR 063518 DI 10.1103/PhysRevD.91.063518 PG 11 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CD8KQ UT WOS:000351344100002 ER PT J AU Nazikian, R Paz-Soldan, C Callen, JD Degrassie, JS Eldon, D Evans, TE Ferraro, NM Grierson, BA Groebner, RJ Haskey, SR Hegna, CC King, JD Logan, NC Mckee, GR Moyer, RA Okabayashi, M Orlov, DM Osborne, TH Park, JK Rhodes, TL Shafer, MW Snyder, PB Solomon, WM Strait, EJ Wade, MR AF Nazikian, R. Paz-Soldan, C. Callen, J. D. Degrassie, J. S. Eldon, D. Evans, T. E. Ferraro, N. M. Grierson, B. A. Groebner, R. J. Haskey, S. R. Hegna, C. C. King, J. D. Logan, N. C. Mckee, G. R. Moyer, R. A. Okabayashi, M. Orlov, D. M. Osborne, T. H. Park, J-K. Rhodes, T. L. Shafer, M. W. Snyder, P. B. Solomon, W. M. Strait, E. J. Wade, M. R. TI Pedestal Bifurcation and Resonant Field Penetration at the Threshold of Edge-Localized Mode Suppression in the DIII-D Tokamak SO PHYSICAL REVIEW LETTERS LA English DT Article ID MAGNETIC PERTURBATIONS; REGIME AB Rapid bifurcations in the plasma response to slowly varying n = 2 magnetic fields are observed as the plasma transitions into and out of edge-localized mode (ELM) suppression. The rapid transition to ELM suppression is characterized by an increase in the toroidal rotation and a reduction in the electron pressure gradient at the top of the pedestal that reduces the perpendicular electron flow there to near zero. These events occur simultaneously with an increase in the inner-wall magnetic response. These observations are consistent with strong resonant field penetration of n = 2 fields at the onset of ELM suppression, based on extended MHD simulations using measured plasma profiles. Spontaneous transitions into (and out of) ELM suppression with a static applied n = 2 field indicate competing mechanisms of screening and penetration of resonant fields near threshold conditions. Magnetic measurements reveal evidence for the unlocking and rotation of tearinglike structures as the plasma transitions out of ELM suppression. C1 [Nazikian, R.; Grierson, B. A.; Logan, N. C.; Okabayashi, M.; Park, J-K.; Solomon, W. M.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. [Paz-Soldan, C.; Degrassie, J. S.; Evans, T. E.; Ferraro, N. M.; Groebner, R. J.; King, J. D.; Osborne, T. H.; Snyder, P. B.; Strait, E. J.; Wade, M. R.] Gen Atom Co, San Diego, CA 92186 USA. [Eldon, D.; Moyer, R. A.; Orlov, D. M.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Haskey, S. R.] Australian Natl Univ, Plasma Res Lab, Canberra, ACT 0200, Australia. [Callen, J. D.; Hegna, C. C.; Mckee, G. R.] Univ Wisconsin, Madison, WI 53706 USA. [Rhodes, T. L.] Univ Calif Los Angeles, Los Angeles, CA 90095 USA. [Shafer, M. W.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Nazikian, R (reprint author), Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA. EM rnazikian@pppl.gov RI Haskey, Shaun/M-1469-2015; Orlov, Dmitriy/D-2406-2016; OI Haskey, Shaun/0000-0002-9978-6597; Orlov, Dmitriy/0000-0002-2230-457X; Solomon, Wayne/0000-0002-0902-9876; Eldon, David/0000-0003-1895-0648 FU U.S. Department of Energy [DE-FC02-04ER54698, DE-AC02-09CH11466, DE-FG02-07ER54917, DE-FG02-89ER53296, DE-FG02-08ER54999, DE-FG02-08ER54984, DE-AC05-00OR22725, DE-FG02-86ER53218, DE-FG02-92ER54139] FX This work is supported by the U.S. Department of Energy under Awards No. DE-FC02-04ER54698, No. DE-AC02-09CH11466, No. DE-FG02-07ER54917, No. DE-FG02-89ER53296, No. DE-FG02-08ER54999, No. DE-FG02-08ER54984, No. DE-AC05-00OR22725, No. DE-FG02-86ER53218, and No. DE-FG02-92ER54139. NR 22 TC 23 Z9 23 U1 5 U2 33 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 12 PY 2015 VL 114 IS 10 AR 105002 DI 10.1103/PhysRevLett.114.105002 PG 5 WC Physics, Multidisciplinary SC Physics GA CD8LZ UT WOS:000351347800004 PM 25815938 ER PT J AU Paz-Soldan, C Nazikian, R Haskey, SR Logan, NC Strait, EJ Ferraro, NM Hanson, JM King, JD Lanctot, MJ Moyer, RA Okabayashi, M Park, JK Shafer, MW Tobias, BJ AF Paz-Soldan, C. Nazikian, R. Haskey, S. R. Logan, N. C. Strait, E. J. Ferraro, N. M. Hanson, J. M. King, J. D. Lanctot, M. J. Moyer, R. A. Okabayashi, M. Park, J-K. Shafer, M. W. Tobias, B. J. TI Observation of a Multimode Plasma Response and its Relationship to Density Pumpout and Edge-Localized Mode Suppression SO PHYSICAL REVIEW LETTERS LA English DT Article AB Density pumpout and edge-localized mode (ELM) suppression by applied n = 2 magnetic fields in low-collisionality DIII-D plasmas are shown to be correlated with the magnitude of the plasma response driven on the high-field side (HFS) of the magnetic axis but not the low-field side (LFS) midplane. These distinct responses are a direct measurement of a multimodal magnetic plasma response, with each structure preferentially excited by a different n = 2 applied spectrum and preferentially detected on the LFS or HFS. Ideal and resistive magneto-hydrodynamic (MHD) calculations find that the LFS measurement is primarily sensitive to the excitation of stable kink modes, while the HFS measurement is primarily sensitive to resonant currents (whether fully shielding or partially penetrated). The resonant currents are themselves strongly modified by kink excitation, with the optimal applied field pitch for pumpout and ELM suppression significantly differing from equilibrium field alignment. C1 [Paz-Soldan, C.; Strait, E. J.; Ferraro, N. M.; King, J. D.; Lanctot, M. J.] Gen Atom Co, San Diego, CA 92121 USA. [Nazikian, R.; Logan, N. C.; Okabayashi, M.; Park, J-K.; Tobias, B. J.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. [Haskey, S. R.] Australian Natl Univ, Plasma Res Lab, Canberra, ACT 0200, Australia. [Hanson, J. M.] Columbia Univ, New York, NY 10027 USA. [Moyer, R. A.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Shafer, M. W.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Paz-Soldan, C (reprint author), Gen Atom Co, San Diego, CA 92121 USA. EM paz-soldan@fusion.gat.com RI Haskey, Shaun/M-1469-2015; Lanctot, Matthew J/O-4979-2016 OI Haskey, Shaun/0000-0002-9978-6597; Lanctot, Matthew J/0000-0002-7396-3372 FU U.S. Department of Energy, Office of Science, Office of Fusion Energy Sciences [DE-FC02-04ER54698, DE-AC02-09CH11466, DE-FG02-04ER54761, DE-AC05-06OR23100, DE-SC0001961, DE-AC05-00OR22725]; AINSE; ANSTO FX This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Fusion Energy Sciences, using the DIII-D National Fusion Facility, a DOE Office of Science user facility, under Awards No. DE-FC02-04ER54698, No. DE-AC02-09CH11466, No. DE-FG02-04ER54761, No. DE-AC05-06OR23100, No. DE-SC0001961, and No. DE-AC05-00OR22725. S. R. H. was supported by AINSE and ANSTO. NR 26 TC 22 Z9 22 U1 5 U2 17 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 12 PY 2015 VL 114 IS 10 AR 105001 DI 10.1103/PhysRevLett.114.105001 PG 5 WC Physics, Multidisciplinary SC Physics GA CD8LZ UT WOS:000351347800003 PM 25815937 ER PT J AU Wlazlowski, G Bulgac, A Forbes, MM Roche, KJ AF Wlazlowski, Gabriel Bulgac, Aurel Forbes, Michael McNeil Roche, Kenneth J. TI Life cycle of superfluid vortices and quantum turbulence in the unitary Fermi gas SO PHYSICAL REVIEW A LA English DT Article AB The unitary Fermi gas (UFG) offers a unique opportunity to study quantum turbulence both experimentally and theoretically in a strongly interacting fermionic superfluid with the highest vortex line density of any known superfluid. It yields to accurate and controlled experiments and admits the only dynamical microscopic description via time-dependent density-functional theory, apart from dilute bosonic gases, of the crossing and reconnection of superfluid vortex lines conjectured by Feynman [R. P. Feynman, Prog. Low Temp. Phys. 1, 17 (1955)] to be at the origin of quantum turbulence in superfluids at zero temperature. We demonstrate how various vortex configurations can be generated by using well-established experimental techniques: laser stirring and phase imprinting. New imaging techniques demonstrated by Ku et al. [M. J. H. Ku et al., Phys. Rev. Lett. 113, 065301 (2014)] should be able to directly visualize these crossings and reconnections in greater detail than performed so far in liquid helium. We demonstrate the critical role played by the geometry of the trap in the formation and dynamics of a vortex in the UFG and how laser stirring and phase imprint can be used to create vortex tangles with clear signatures of the onset of quantum turbulence. C1 [Wlazlowski, Gabriel] Warsaw Univ Technol, Fac Phys, PL-00662 Warsaw, Poland. [Wlazlowski, Gabriel; Bulgac, Aurel; Forbes, Michael McNeil; Roche, Kenneth J.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Forbes, Michael McNeil] Washington State Univ, Dept Phys & Astron, Pullman, WA 99164 USA. [Forbes, Michael McNeil] Univ Washington, Inst Nucl Theory, Seattle, WA 98195 USA. [Roche, Kenneth J.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Wlazlowski, G (reprint author), Warsaw Univ Technol, Fac Phys, Koszykowa 75, PL-00662 Warsaw, Poland. EM gabrielw@if.pw.edu.pl; bulgac@uw.edu; mforbes@alum.mit.edu; k8r@u.washington.edu FU U.S. Department of Energy (DOE) [DE-FG02-97ER41014]; Polish National Science Center [DEC-2013/08/A/ST3/00708]; Center for Advanced Studies at Warsaw University of Technology (European Union from the European Social Funds) [58/2013, CAS/32/POKL]; Institute for Nuclear Theory [INT-14-1]; NSF MRI [PHY-0922770]; Office of Science of the DOE [DE-AC05-00OR22725] FX We thank L. Chuek, M. Ku, and M. Zwierlein for describing details of their experiment. We acknowledge support under U.S. Department of Energy (DOE) Grant No. DE-FG02-97ER41014 and the Polish National Science Center grant under decision No. DEC-2013/08/A/ST3/00708. G.W. acknowledges the Center for Advanced Studies at Warsaw University of Technology for support under Contract No. 58/2013 (international research scholarships financed by the European Union from the European Social Funds CAS/32/POKL). M.M.F. acknowledges support from the Institute for Nuclear Theory during the program Universality in Few-Body Systems: Theoretical Challenges and New Directions, INT-14-1. Some of the calculations reported here were performed at the University of Washington Hyak cluster funded by the NSF MRI Grant No. PHY-0922770. This research also used resources of the National Center for Computational Sciences at Oak Ridge National Laboratory [35], which is supported by the Office of Science of the DOE under Contract No. DE-AC05-00OR22725. NR 36 TC 7 Z9 7 U1 3 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1050-2947 EI 1094-1622 J9 PHYS REV A JI Phys. Rev. A PD MAR 12 PY 2015 VL 91 IS 3 AR 031602 DI 10.1103/PhysRevA.91.031602 PG 5 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA CD8JC UT WOS:000351340100001 ER PT J AU Traverso, JJ Manoranjan, VS Bishop, AR Rasmussen, KO Voulgarakis, NK AF Traverso, Joseph J. Manoranjan, Valipuram S. Bishop, A. R. Rasmussen, Kim O. Voulgarakis, Nikolaos K. TI Allostery through protein-induced DNA bubbles SO SCIENTIFIC REPORTS LA English DT Article ID MITOCHONDRIAL TRANSCRIPTION FACTOR; RNA-POLYMERASE; MODEL; MTDNA; DENATURATION; ORGANIZATION; COMPONENT; PROMOTER; BINDING; FORCES AB Allostery through DNA is increasingly recognized as an important modulator of DNA functions. Here, we show that the coalescence of protein-induced DNA bubbles can mediate allosteric interactions that drive protein aggregation. We propose that such allostery may regulate DNA's flexibility and the assembly of the transcription machinery. Mitochondrial transcription factor A (TFAM), a dual-function protein involved in mitochondrial DNA (mtDNA) packaging and transcription initiation, is an ideal candidate to test such a hypothesis owing to its ability to locally unwind the double helix. Numerical simulations demonstrate that the coalescence of TFAM-induced bubbles can explain experimentally observed TFAM oligomerization. The resulting melted DNA segment, approximately 10 base pairs long, around the joints of the oligomers act as flexible hinges, which explains the efficiency of TFAM in compacting DNA. Since mitochondrial polymerase (mitoRNAP) is involved in melting the transcription bubble, TFAM may use the same allosteric interaction to both recruit mitoRNAP and initiate transcription. C1 [Traverso, Joseph J.; Voulgarakis, Nikolaos K.] Washington State Univ, Dept Math, Richland, WA 99354 USA. [Traverso, Joseph J.] Washington State Univ, Dept Mech Engn, Richland, WA 99354 USA. [Manoranjan, Valipuram S.] Washington State Univ, Dept Math, Pullman, WA 99163 USA. [Bishop, A. R.; Rasmussen, Kim O.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Voulgarakis, NK (reprint author), Washington State Univ, Dept Math, Richland, WA 99354 USA. EM n.voulgarakis@wsu.edu RI Rasmussen, Kim/B-5464-2009 OI Rasmussen, Kim/0000-0002-4029-4723 FU Washington State University FX J.J.T. acknowledges support from Auvil and Carson fellowships of Washington State University. NR 43 TC 3 Z9 3 U1 1 U2 11 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAR 12 PY 2015 VL 5 AR 9037 DI 10.1038/srep09037 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CD5RG UT WOS:000351144900014 PM 25762409 ER PT J AU Nunez, JK Lee, ASY Engelman, A Doudna, JA AF Nunez, James K. Lee, Amy S. Y. Engelman, Alan Doudna, Jennifer A. TI Integrase-mediated spacer acquisition during CRISPR-Cas adaptive immunity SO NATURE LA English DT Article ID HUMAN-IMMUNODEFICIENCY-VIRUS; SHORT PALINDROMIC REPEATS; TOPOISOMERASE-I MUTANTS; DNA STRAND TRANSFER; ESCHERICHIA-COLI; ACQUIRED-RESISTANCE; BACTERIAL IMMUNITY; GYRASE GENES; SEQUENCE; SYSTEM AB Bacteria and archaea insert spacer sequences acquired from foreign DNAs into CRISPR loci to generate immunological memory. The Escherichia coli Cas1-Cas2 complex mediates spacer acquisition in vivo, but the molecular mechanism of this process is unknown. Here we show that the purified Cas1-Cas2 complex integrates oligonucleotide DNA substrates into acceptor DNA to yield products similar to those generated by retroviral integrases and transposases. Cas1 is the catalytic subunit and Cas2 substantially increases integration activity. Protospacer DNA with free 3'-OH ends and supercoiled target DNA are required, and integration occurs preferentially at the ends of CRISPR repeats and at sequences adjacent to cruciform structures abutting AT-rich regions, similar to the CRISPR leader sequence. Our results demonstrate the Cas1-Cas2 complex to be the minimal machinery that catalyses spacer DNA acquisition and explain the significance of CRISPR repeats in providing sequence and structural specificity for Cas1-Cas2-mediated adaptive immunity. C1 [Nunez, James K.; Lee, Amy S. Y.; Doudna, Jennifer A.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Lee, Amy S. Y.; Doudna, Jennifer A.] Univ Calif Berkeley, Ctr RNA Syst Biol, Berkeley, CA 94720 USA. [Engelman, Alan] Harvard Univ, Sch Med, Dana Farber Canc Inst, Dept Canc Immunol & AIDS, Boston, MA 02115 USA. [Engelman, Alan] Harvard Univ, Sch Med, Dept Med, Boston, MA 02115 USA. [Doudna, Jennifer A.] Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA. [Doudna, Jennifer A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Doudna, Jennifer A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Doudna, JA (reprint author), Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA. EM doudna@berkeley.edu FU US National Science Foundation [1244557]; NIH [AI070042]; NIH S10 Instrumentation Grants [S10RR029668, S10RR027303]; US National Science Foundation Graduate Research Fellowship; UC Berkeley Chancellor's Graduate Fellowship; American Cancer Society [PF-14-108-01-RMC] FX We are grateful to M. Chung, P. J. Kranzusch and A.V. Wright for technical assistance and members of the Doudna laboratory and J. Cate for discussions. This project was funded by US National Science Foundation grant no. 1244557 to J.A.D. and by NIH grant AI070042 to A.E. This work used the Vincent J. Coates Genomics Sequencing Laboratory at UC Berkeley, supported by NIH S10 Instrumentation Grants S10RR029668 and S10RR027303. J.K.N. is supported by a US National Science Foundation Graduate Research Fellowship and a UC Berkeley Chancellor's Graduate Fellowship. A.S.Y.L. is supported as an American Cancer Society Postdoctoral Fellow (PF-14-108-01-RMC). J.A.D. is an Investigator of the Howard Hughes Medical Institute and a member of the Center for RNA Systems Biology. NR 49 TC 66 Z9 69 U1 8 U2 68 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD MAR 12 PY 2015 VL 519 IS 7542 BP 193 EP + DI 10.1038/nature14237 PG 17 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CD0NH UT WOS:000350770500030 PM 25707795 ER PT J AU Aartsen, MG Ackermann, M Adams, J Aguilar, JA Ahlers, M Ahrens, M Altmann, D Anderson, T Arguelles, C Arlen, TC Auffenberg, J Bai, X Barwick, SW Baum, V Beatty, JJ Tjus, JB Becker, KH BenZvi, S Berghaus, P Berley, D Bernardini, E Bernhard, A Besson, DZ Binder, G Bindig, D Bissok, M Blaufuss, E Blumenthal, J Boersma, DJ Bohm, C Bos, F Bose, D Boeser, S Botner, O Brayeur, L Bretz, HP Brown, AM Casey, J Casier, M Cheung, E Chirkin, D Christov, A Christy, B Clark, K Classen, L Clevermann, F Coenders, S Cowen, DF Silva, AHC Danninger, M Daughhetee, J Davis, JC Day, M De Andre, JPAM DeClercq, C De Ridder, S Desiati, P De Vries, KD Dewith, M DeYoung, T Diaz-Velez, JC Dunkman, M Eagan, R Eberhardt, B Eichmann, B Eisch, J Euler, S Evenson, PA Fadiran, O Fazely, AR Fedynitch, A Feintzeig, J Felde, J Feusels, T Filimonov, K Finley, C Fischer-Wasels, T Flis, S Franckowiak, A Frantzen, K Fuchs, T Gaisser, TK Gaior, R Gallagher, J Gerhardt, L Gier, D Gladstone, L Glusenkamp, T Goldschmidt, A Golup, G Gonzalez, JG Goodman, JA Gora, D Grant, D Gretskov, P Groh, JC Gro, A Ha, C Haack, C Ismail, AH Hallen, P Hallgren, A Halzen, F Hanson, K Hebecker, D Heereman, D Heinen, D Helbing, K Hellauer, R Hellwig, D Hickford, S Hill, GC Hoffman, KD Hoffmann, R Homeier, A Hoshina, K Huang, F Huelsnitz, W Hulth, PO Hultqvist, K Hussain, S Ishihara, A Jacobi, E Jacobsen, J Jagielski, K Japaridze, GS Jero, K Jlelati, O Jurkovic, M Kaminsky, B Kappes, A Karg, T Karle, A Kauer, M Keivani, A Kelley, JL Kheirandish, A Kiryluk, J Klaes, J Klein, SR Koehne, JH Kohnen, G Kolanoski, H Koob, A Koepke, L Kopper, C Kopper, S Koskinen, DJ Kowalski, M Kriesten, A Krings, K Kroll, G Kroll, M Kunnen, J Kurahashi, N Kuwabara, T Labare, M Larsen, DT Larson, MJ Lesiak-Bzdak, M Leuermann, M Leute, J Luenemann, J Madsen, J Maggi, G Maruyama, R Mase, K Matis, HS Maunu, R McNally, F Meagher, K Medici, M Meli, A Meures, T Miarecki, S Middell, E Middlemas, E Milke, N Miller, J Mohrmann, L Montaruli, T Morse, R Nahnhauer, R Naumann, U Niederhausen, H Nowicki, SC Nygren, DR Obertacke, A Odrowski, S Olivas, A Omairat, A O'Murchadha, A Palczewski, T Paul, L Penek, O Pepper, JA Heros, CPDL Pfendner, C Pieloth, D Pinat, E Posselt, J Price, PB Przybylski, GT Puetz, J Quinnan, M Raedel, L Rameez, M Rawlins, K Redl, P Rees, I Reimann, R Relich, M Resconi, E Rhode, W Richman, M Riedel, B Robertson, S Rodrigues, JP Rongen, M Rott, C Ruhe, T Ruzybayev, B Ryckbosch, D Saba, SM Sander, HG Sandroos, J Santander, M Sarkar, S Schatto, K Scheriau, F Schmidt, T Schmitz, M Schoenen, S Schoeneberg, S Schoenwald, A Schukraft, A Schulte, L Schulz, O Seckel, D Sestayo, Y Seunarine, S Shanidze, R Smith, MWE Soldin, D Spiczak, GM Spiering, C Stamatikos, M Stanev, T Stanisha, NA Stasik, A Stezelberger, T Stokstad, RG Stoessl, A Strahler, EA Stroem, R Strotjohann, NL Sullivan, GW Taavola, H Taboada, I Tamburro, A Tepe, A Ter-Antonyan, S Terliuk, A Tesic, G Tilav, S Toale, PA Tobin, MN Tosi, D Tselengidou, M Unger, E Usner, M Vallecorsa, S Van Eijndhoven, N Vandenbroucke, J Van Santen, J Vehring, M Voge, M Vraeghe, M Walck, C Wallraff, M Weaver, C Wellons, M Wendt, C Westerhoff, S Whelan, BJ Whitehorn, N Wichary, C Wiebe, K Wiebusch, CH Williams, DR Wissing, H Wolf, M Wood, TR Woschnagg, K Xu, DL Xu, XW Yanez, JP Yodh, G Yoshida, S Zarzhitsky, P Ziemann, J Zierke, S Zoll, M Morik, K AF Aartsen, M. G. Ackermann, M. Adams, J. Aguilar, J. A. Ahlers, M. Ahrens, M. Altmann, D. Anderson, T. Arguelles, C. Arlen, T. C. Auffenberg, J. Bai, X. Barwick, S. W. Baum, V. Beatty, J. J. Tjus, J. Becker Becker, K. -H. BenZvi, S. Berghaus, P. Berley, D. Bernardini, E. Bernhard, A. Besson, D. Z. Binder, G. Bindig, D. Bissok, M. Blaufuss, E. Blumenthal, J. Boersma, D. J. Bohm, C. Bos, F. Bose, D. Boeser, S. Botner, O. Brayeur, L. Bretz, H. P. Brown, A. M. Casey, J. Casier, M. Cheung, E. Chirkin, D. Christov, A. Christy, B. Clark, K. Classen, L. Clevermann, F. Coenders, S. Cowen, D. F. Silva, A. H. Cruz Danninger, M. Daughhetee, J. Davis, J. C. Day, M. De Andre, J. P. A. M. DeClercq, C. De Ridder, S. Desiati, P. De Vries, K. D. Dewith, M. DeYoung, T. Diaz-Velez, J. C. Dunkman, M. Eagan, R. Eberhardt, B. Eichmann, B. Eisch, J. Euler, S. Evenson, P. A. Fadiran, O. Fazely, A. R. Fedynitch, A. Feintzeig, J. Felde, J. Feusels, T. Filimonov, K. Finley, C. Fischer-Wasels, T. Flis, S. Franckowiak, A. Frantzen, K. Fuchs, T. Gaisser, T. K. Gaior, R. Gallagher, J. Gerhardt, L. Gier, D. Gladstone, L. Glusenkamp, T. Goldschmidt, A. Golup, G. Gonzalez, J. G. Goodman, J. A. Gora, D. Grant, D. Gretskov, P. Groh, J. C. Gro, A. Ha, C. Haack, C. Ismail, A. Haj Hallen, P. Hallgren, A. Halzen, F. Hanson, K. Hebecker, D. Heereman, D. Heinen, D. Helbing, K. Hellauer, R. Hellwig, D. Hickford, S. Hill, G. C. Hoffman, K. D. Hoffmann, R. Homeier, A. Hoshina, K. Huang, F. Huelsnitz, W. Hulth, P. O. Hultqvist, K. Hussain, S. Ishihara, A. Jacobi, E. Jacobsen, J. Jagielski, K. Japaridze, G. S. Jero, K. Jlelati, O. Jurkovic, M. Kaminsky, B. Kappes, A. Karg, T. Karle, A. Kauer, M. Keivani, A. Kelley, J. L. Kheirandish, A. Kiryluk, J. Klaes, J. Klein, S. R. Koehne, J. H. Kohnen, G. Kolanoski, H. Koob, A. Koepke, L. Kopper, C. Kopper, S. Koskinen, D. J. Kowalski, M. Kriesten, A. Krings, K. Kroll, G. Kroll, M. Kunnen, J. Kurahashi, N. Kuwabara, T. Labare, M. Larsen, D. T. Larson, M. J. Lesiak-Bzdak, M. Leuermann, M. Leute, J. Luenemann, J. Madsen, J. Maggi, G. Maruyama, R. Mase, K. Matis, H. S. Maunu, R. McNally, F. Meagher, K. Medici, M. Meli, A. Meures, T. Miarecki, S. Middell, E. Middlemas, E. Milke, N. Miller, J. Mohrmann, L. Montaruli, T. Morse, R. Nahnhauer, R. Naumann, U. Niederhausen, H. Nowicki, S. C. Nygren, D. R. Obertacke, A. Odrowski, S. Olivas, A. Omairat, A. O'Murchadha, A. Palczewski, T. Paul, L. Penek, Oe. Pepper, J. A. Heros, C. Perez De Los Pfendner, C. Pieloth, D. Pinat, E. Posselt, J. Price, P. B. Przybylski, G. T. Puetz, J. Quinnan, M. Raedel, L. Rameez, M. Rawlins, K. Redl, P. Rees, I. Reimann, R. Relich, M. Resconi, E. Rhode, W. Richman, M. Riedel, B. Robertson, S. Rodrigues, J. P. Rongen, M. Rott, C. Ruhe, T. Ruzybayev, B. Ryckbosch, D. Saba, S. M. Sander, H. -G. Sandroos, J. Santander, M. Sarkar, S. Schatto, K. Scheriau, F. Schmidt, T. Schmitz, M. Schoenen, S. Schoeneberg, S. Schoenwald, A. Schukraft, A. Schulte, L. Schulz, O. Seckel, D. Sestayo, Y. Seunarine, S. Shanidze, R. Smith, M. W. E. Soldin, D. Spiczak, G. M. Spiering, C. Stamatikos, M. Stanev, T. Stanisha, N. A. Stasik, A. Stezelberger, T. Stokstad, R. G. Stoessl, A. Strahler, E. A. Stroem, R. Strotjohann, N. L. Sullivan, G. W. Taavola, H. Taboada, I. Tamburro, A. Tepe, A. Ter-Antonyan, S. Terliuk, A. Tesic, G. Tilav, S. Toale, P. A. Tobin, M. N. Tosi, D. Tselengidou, M. Unger, E. Usner, M. Vallecorsa, S. Van Eijndhoven, N. Vandenbroucke, J. Van Santen, J. Vehring, M. Voge, M. Vraeghe, M. Walck, C. Wallraff, M. Weaver, Ch. Wellons, M. Wendt, C. Westerhoff, S. Whelan, B. J. Whitehorn, N. Wichary, C. Wiebe, K. Wiebusch, C. H. Williams, D. R. Wissing, H. Wolf, M. Wood, T. R. Woschnagg, K. Xu, D. L. Xu, X. W. Yanez, J. P. Yodh, G. Yoshida, S. Zarzhitsky, P. Ziemann, J. Zierke, S. Zoll, M. Morik, K. CA IceCube Collaboration TI Development of a general analysis and unfolding scheme and its application to measure the energy spectrum of atmospheric neutrinos with IceCube SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID 200 TEV; TELESCOPE; DETECTOR; PERFORMANCE; AMANDA; SYSTEM AB We present the development and application of a generic analysis scheme for the measurement of neutrino spectra with the IceCube detector. This scheme is based on regularized unfolding, preceded by an event selection which uses a Minimum Redundancy Maximum Relevance algorithm to select the relevant variables and a random forest for the classification of events. The analysis has been developed using IceCube data from the 59-string configuration of the detector. 27,771 neutrino candidates were detected in 346 days of livetime. A rejection of 99.9999 % of the atmospheric muon background is achieved. The energy spectrum of the atmospheric neutrino flux is obtained using the TRUEE unfolding program. The unfolded spectrum of atmospheric muon neutrinos covers an energy range from 100 GeV to 1 PeV. Compared to the previous measurement using the detector in the 40-string configuration, the analysis presented here, extends the upper end of the atmospheric neutrino spectrum by more than a factor of two, reaching an energy region that has not been previously accessed by spectral measurements. C1 [Auffenberg, J.; Bissok, M.; Blumenthal, J.; Fedynitch, A.; Franckowiak, A.; Gier, D.; Gretskov, P.; Haack, C.; Hallen, P.; Heinen, D.; Hellwig, D.; Jagielski, K.; Koob, A.; Kriesten, A.; Krings, K.; Leuermann, M.; Paul, L.; Penek, Oe.; Puetz, J.; Raedel, L.; Reimann, R.; Rongen, M.; Schoenen, S.; Schukraft, A.; Vehring, M.; Wallraff, M.; Wichary, C.; Wiebusch, C. H.; Zierke, S.] Rhein Westfal TH Aachen, Inst Phys 3, D-52056 Aachen, Germany. [Aartsen, M. G.; Hill, G. C.; Robertson, S.; Whelan, B. J.] Univ Adelaide, Sch Chem & Phys, Adelaide, SA 5005, Australia. [Rawlins, K.] Univ Alaska Anchorage, Dept Phys & Astron, Anchorage, AK 99508 USA. [Japaridze, G. S.] Clark Atlanta Univ, CTSPS, Atlanta, GA 30314 USA. [Casey, J.; Daughhetee, J.; Taboada, I.] Georgia Inst Technol, Sch Phys, Atlanta, GA 30332 USA. [Casey, J.; Daughhetee, J.; Taboada, I.] Georgia Inst Technol, Ctr Relativist Astrophys, Atlanta, GA 30332 USA. [Fazely, A. R.; Ter-Antonyan, S.; Xu, X. W.] Southern Univ, Dept Phys, Baton Rouge, LA 70813 USA. [Binder, G.; Filimonov, K.; Gerhardt, L.; Ha, C.; Klein, S. R.; Miarecki, S.; Price, P. B.; Woschnagg, K.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Binder, G.; Gerhardt, L.; Goldschmidt, A.; Ha, C.; Klein, S. R.; Matis, H. S.; Miarecki, S.; Nygren, D. R.; Przybylski, G. T.; Stezelberger, T.; Stokstad, R. G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Dewith, M.; Kolanoski, H.] Humboldt Univ, Inst Phys, D-12489 Berlin, Germany. [Tjus, J. Becker; Bos, F.; Eichmann, B.; Fedynitch, A.; Kroll, M.; Saba, S. M.; Schoeneberg, S.] Ruhr Univ Bochum, Fak Phys & Astron, D-44780 Bochum, Germany. [Boeser, S.; Franckowiak, A.; Hebecker, D.; Homeier, A.; Kowalski, M.; Schulte, L.; Stasik, A.; Strotjohann, N. L.; Usner, M.; Voge, M.] Univ Bonn, Phys Inst, D-53115 Bonn, Germany. [Hanson, K.; Heereman, D.; Meures, T.; O'Murchadha, A.; Pinat, E.] Univ Libre Bruxelles, Sci Fac CP230, B-1050 Brussels, Belgium. [Brayeur, L.; Casier, M.; DeClercq, C.; De Vries, K. D.; Golup, G.; Kunnen, J.; Maggi, G.; Miller, J.; Strahler, E. A.; Van Eijndhoven, N.] Vrije Univ Brussel, Dienst ELEM, B-1050 Brussels, Belgium. [Gaior, R.; Ishihara, A.; Kuwabara, T.; Mase, K.; Relich, M.; Yoshida, S.] Chiba Univ, Dept Phys, Chiba 2638522, Japan. [Adams, J.; Brown, A. M.; Hickford, S.] Univ Canterbury, Dept Phys & Astron, Christchurch 1, New Zealand. [Berley, D.; Blaufuss, E.; Cheung, E.; Christy, B.; Felde, J.; Goodman, J. A.; Hellauer, R.; Hoffman, K. D.; Huelsnitz, W.; Maunu, R.; Meagher, K.; Olivas, A.; Redl, P.; Richman, M.; Schmidt, T.; Sullivan, G. W.; Wissing, H.] Univ Maryland, Dept Phys, College Pk, MD 20742 USA. [Beatty, J. J.; Davis, J. C.; Pfendner, C.; Stamatikos, M.] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. [Beatty, J. J.; Davis, J. C.; Pfendner, C.; Stamatikos, M.] Ohio State Univ, Ctr Cosmol & Astroparticle Phys, Columbus, OH 43210 USA. [Beatty, J. J.] Ohio State Univ, Dept Astron, Columbus, OH 43210 USA. [Koskinen, D. J.; Larson, M. J.; Medici, M.; Sandroos, J.; Sarkar, S.] Univ Copenhagen, Niels Bohr Inst, DK-2100 Copenhagen, Denmark. [Clevermann, F.; Frantzen, K.; Fuchs, T.; Koehne, J. H.; Milke, N.; Pieloth, D.; Rhode, W.; Ruhe, T.; Scheriau, F.; Schmitz, M.; Ziemann, J.] TU Dortmund Univ, Dept Phys, D-44221 Dortmund, Germany. [Morik, K.] TU Dortmund Univ, Dept Comp Sci, D-44221 Dortmund, Germany. [Grant, D.; Nowicki, S. C.; Odrowski, S.; Wood, T. R.] Univ Alberta, Dept Phys, Edmonton, AB T6G 2E1, Canada. [Altmann, D.; Classen, L.; Kappes, A.; Tselengidou, M.] Univ Erlangen Nurnberg, Erlangen Ctr Astroparticle Phys, D-91058 Erlangen, Germany. [Aguilar, J. A.; Christov, A.; Montaruli, T.; Rameez, M.; Vallecorsa, S.] Univ Geneva, Dept Phys Nucl & Corpusculaire, CH-1211 Geneva, Switzerland. [De Ridder, S.; Feusels, T.; Ismail, A. Haj; Jlelati, O.; Labare, M.; Meli, A.; Ryckbosch, D.; Vraeghe, M.] Univ Ghent, Dept Phys & Astron, B-9000 Ghent, Belgium. [Barwick, S. W.; Day, M.; Yodh, G.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. [Besson, D. Z.] Univ Kansas, Dept Phys & Astron, Lawrence, KS 66045 USA. [Gallagher, J.] Univ Wisconsin, Dept Astron, Madison, WI 53706 USA. [Ahlers, M.; Arguelles, C.; BenZvi, S.; Chirkin, D.; Desiati, P.; Diaz-Velez, J. C.; Eisch, J.; Fadiran, O.; Feintzeig, J.; Gladstone, L.; Halzen, F.; Hoshina, K.; Jacobsen, J.; Jero, K.; Karle, A.; Kauer, M.; Kelley, J. L.; Kheirandish, A.; Kopper, C.; Kurahashi, N.; Larsen, D. T.; Maruyama, R.; McNally, F.; Middlemas, E.; Morse, R.; Rees, I.; Riedel, B.; Rodrigues, J. P.; Santander, M.; Tobin, M. N.; Tosi, D.; Vandenbroucke, J.; Van Santen, J.; Weaver, Ch.; Wellons, M.; Wendt, C.; Westerhoff, S.; Whitehorn, N.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Ahlers, M.; Arguelles, C.; BenZvi, S.; Chirkin, D.; Desiati, P.; Diaz-Velez, J. C.; Eisch, J.; Fadiran, O.; Feintzeig, J.; Gladstone, L.; Halzen, F.; Hoshina, K.; Jacobsen, J.; Jero, K.; Karle, A.; Kauer, M.; Kelley, J. L.; Kheirandish, A.; Kopper, C.; Kurahashi, N.; Larsen, D. T.; Maruyama, R.; McNally, F.; Middlemas, E.; Morse, R.; Rees, I.; Riedel, B.; Rodrigues, J. P.; Santander, M.; Tobin, M. N.; Tosi, D.; Vandenbroucke, J.; Van Santen, J.; Weaver, Ch.; Wellons, M.; Wendt, C.; Westerhoff, S.; Whitehorn, N.] Univ Wisconsin, Wisconsin IceCube Particle Astrophys Ctr, Madison, WI 53706 USA. [Baum, V.; Eberhardt, B.; Koepke, L.; Kroll, G.; Luenemann, J.; Sander, H. -G.; Schatto, K.; Wiebe, K.] Johannes Gutenberg Univ Mainz, Inst Phys, D-55099 Mainz, Germany. [Kohnen, G.] Univ Mons, B-7000 Mons, Belgium. [Bernhard, A.; Coenders, S.; Gro, A.; Jurkovic, M.; Leute, J.; Resconi, E.; Schulz, O.; Sestayo, Y.] Tech Univ Munich, D-85738 Garching, Germany. [Evenson, P. A.; Gaisser, T. K.; Gonzalez, J. G.; Hussain, S.; Ruzybayev, B.; Seckel, D.; Stanev, T.; Tamburro, A.; Tilav, S.] Univ Delaware, Bartol Res Inst, Dept Phys & Astron, Newark, DE 19716 USA. [Sarkar, S.] Univ Oxford, Dept Phys, Oxford OX1 3NP, England. [Bai, X.] South Dakota Sch Mines & Technol, Dept Phys, Rapid City, SD 57701 USA. [Madsen, J.; Seunarine, S.; Spiczak, G. M.] Univ Wisconsin, Dept Phys, River Falls, WI 54022 USA. [Ahrens, M.; Bohm, C.; Danninger, M.; Finley, C.; Flis, S.; Hulth, P. O.; Hultqvist, K.; Walck, C.; Wolf, M.; Zoll, M.] Stockholm Univ, Oskar Klein Ctr, Dept Phys, S-10691 Stockholm, Sweden. [Kiryluk, J.; Lesiak-Bzdak, M.; Niederhausen, H.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Bose, D.; Rott, C.] Sungkyunkwan Univ, Dept Phys, Suwon 440746, South Korea. [Clark, K.] Univ Toronto, Dept Phys, Toronto, ON M5S 1A7, Canada. [Palczewski, T.; Pepper, J. A.; Toale, P. A.; Williams, D. R.; Xu, D. L.; Zarzhitsky, P.] Univ Alabama, Dept Phys & Astron, Tuscaloosa, AL 35487 USA. [Cowen, D. F.] Penn State Univ, Dept Astron & Astrophys, University Pk, PA 16802 USA. [Anderson, T.; Arlen, T. C.; Cowen, D. F.; De Andre, J. P. A. M.; DeYoung, T.; Dunkman, M.; Eagan, R.; Gora, D.; Groh, J. C.; Huang, F.; Kaminsky, B.; Keivani, A.; Quinnan, M.; Smith, M. W. E.; Stanisha, N. A.; Stoessl, A.; Tesic, G.] Penn State Univ, Dept Phys, University Pk, PA 16802 USA. [Boersma, D. J.; Botner, O.; Euler, S.; Hallgren, A.; Heros, C. Perez De Los; Stroem, R.; Taavola, H.; Unger, E.] Uppsala Univ, Dept Phys & Astron, S-75120 Uppsala, Sweden. [Becker, K. -H.; Bindig, D.; Fischer-Wasels, T.; Helbing, K.; Hoffmann, R.; Klaes, J.; Kopper, S.; Naumann, U.; Obertacke, A.; Omairat, A.; Posselt, J.; Soldin, D.; Tepe, A.] Univ Wuppertal, Dept Phys, D-42119 Wuppertal, Germany. [Ackermann, M.; Berghaus, P.; Bernardini, E.; Bretz, H. P.; Silva, A. H. Cruz; Glusenkamp, T.; Jacobi, E.; Karg, T.; Middell, E.; Mohrmann, L.; Nahnhauer, R.; Schoenwald, A.; Shanidze, R.; Spiering, C.; Terliuk, A.; Yanez, J. P.] DESY, D-15735 Zeuthen, Germany. RP Aartsen, MG (reprint author), Univ Adelaide, Sch Chem & Phys, Adelaide, SA 5005, Australia. EM tim.ruhe@udo.edu RI Wiebusch, Christopher/G-6490-2012; Taavola, Henric/B-4497-2011; Koskinen, David/G-3236-2014; Aguilar Sanchez, Juan Antonio/H-4467-2015; Maruyama, Reina/A-1064-2013; Tjus, Julia/G-8145-2012; Sarkar, Subir/G-5978-2011; Beatty, James/D-9310-2011 OI Strotjohann, Nora Linn/0000-0002-4667-6730; Wiebusch, Christopher/0000-0002-6418-3008; Taavola, Henric/0000-0002-2604-2810; Koskinen, David/0000-0002-0514-5917; Aguilar Sanchez, Juan Antonio/0000-0003-2252-9514; Ter-Antonyan, Samvel/0000-0002-5788-1369; Schukraft, Anne/0000-0002-9112-5479; Groh, John/0000-0001-9880-3634; Larsen, Dag Toppe/0000-0002-9898-2174; Maruyama, Reina/0000-0003-2794-512X; Sarkar, Subir/0000-0002-3542-858X; Beatty, James/0000-0003-0481-4952 FU SCOAP3 FX Funded by SCOAP3 / License Version CC BY 4.0. NR 32 TC 8 Z9 8 U1 0 U2 11 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD MAR 11 PY 2015 VL 75 IS 3 AR 116 DI 10.1140/epjc/s10052-015-3330-z PG 14 WC Physics, Particles & Fields SC Physics GA CJ7HR UT WOS:000355666000004 ER PT J AU Ye, LH Lv, WQ Cui, JY Liang, YC Wu, P Wang, XN He, H Lin, SJ Wang, W Dickerson, JH He, WD AF Ye, Luhan Lv, Weiqiang Cui, Junyi Liang, Yachun Wu, Peng Wang, Xiaoning He, Han Lin, Senjun Wang, Wei Dickerson, James H. He, Weidong TI Lithium-Air Batteries: Performance Interplays with Instability Factors SO CHEMELECTROCHEM LA English DT Review DE electrochemistry; electrode; electrolyte; instability factors; lithium-air batteries ID NONAQUEOUS LI-O-2 BATTERIES; OXIDE FUEL-CELLS; DOPED CARBON NANOTUBES; OXYGEN REDUCTION; DIFFUSIVITY MEASUREMENT; CONCENTRATION-POLARIZATION; DISCHARGE PERFORMANCE; CYCLIC STABILITY; LI/AIR BATTERIES; POROUS GRAPHENE AB Lithium-air batteries are considered to be promising electro-chemical storage devices, due to their high specific energy density. However, instability limits their cyclic performance and rate capacity and also leads to a high overpotential; lithiumair batteries are typically characterized by capacity degradation and short cycle life. Such challenges prevent lithium-air batteries from entering and competing in the battery market. Electrodes, organic solvents, the interface between electrolyte and cathode, and ambient conditions have all been demonstrated to impact substantially the stability of the lithium-air battery. In this Minireview, we focus on electrode and electrolyte decomposition, side reactions, and physical mass transport in aprotic lithium-air batteries, as well as other types of lithiumair batteries, and aim to understand comprehensively their performance and association with instability factors. C1 [Ye, Luhan; Lv, Weiqiang; Cui, Junyi; Liang, Yachun; Wu, Peng; Wang, Xiaoning; He, Han; He, Weidong] Univ Elect Sci & Technol China, Sch Energy Sci & Engn, Chengdu 611731, Sichuan, Peoples R China. [Lin, Senjun] Zhejiang Univ Technol, Dept Ind Design, Hangzhou 310014, Zhejiang, Peoples R China. [Wang, Wei] Harbin Inst Technol, Shenzhen Grad Sch, Dept Mat Sci & Engn, Shenzhen 518055, Peoples R China. [Dickerson, James H.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Dickerson, James H.] Brown Univ, Dept Phys, Providence, RI 02912 USA. [He, Weidong] Vanderbilt Univ, Interdisciplinary Program Mat Sci, Nashville, TN 37234 USA. [He, Weidong] Vanderbilt Univ, Vanderbilt Inst Nanoscale Sci & Engn, Nashville, TN 37234 USA. RP Ye, LH (reprint author), Univ Elect Sci & Technol China, Sch Energy Sci & Engn, Chengdu 611731, Sichuan, Peoples R China. EM weidong.he@uestc.edu.cn NR 102 TC 5 Z9 5 U1 18 U2 185 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 2196-0216 J9 CHEMELECTROCHEM JI ChemElectroChem PD MAR 11 PY 2015 VL 2 IS 3 BP 312 EP 323 DI 10.1002/celc.201402315 PG 12 WC Electrochemistry SC Electrochemistry GA CD7UD UT WOS:000351298300001 ER PT J AU Kim, JK Lee, E Kim, H Johnson, C Cho, J Kim, Y AF Kim, Jae-Kwang Lee, Eungje Kim, Hyojin Johnson, Christopher Cho, Jaephil Kim, Youngsik TI Rechargeable Seawater Battery and Its Electrochemical Mechanism SO CHEMELECTROCHEM LA English DT Article DE electrochemistry; energy storage; green chemistry; seawater cathode material; sodium ID ION BATTERIES; ELECTROLYTE; SODIUM; REACTIVITY; INSERTION; LITHIUM; NASICON; WATER AB Herein, we explore the electrochemical mechanism of a novel rechargeable seawater battery system that uses seawater as the cathode material. Sodium is harvested from seawater while charging the battery, and the harvested sodium is discharged with oxygen dissolved in the seawater, functioning as oxidants to produce electricity. The seawater provides both anode (Na metal) and cathode (O-2) materials for the proposed battery. Based on the discharge voltage (-2.9 V) with participation of O-2 and the charge voltage (similar to 4.1 V) with Cl-2 evolution during the first cycle, a voltage efficiency of about 73% is obtained. If the seawater battery is constructed using hard carbon as the anode and a Na super ion conductor as the solid electrolyte, a strong cycle performance of 84% is observed after 40 cycles. C1 [Kim, Jae-Kwang; Kim, Hyojin; Cho, Jaephil; Kim, Youngsik] Ulsan Natl Inst Sci & Technol, Dept Energy & Chem Engn, Ulsan 689798, South Korea. [Lee, Eungje; Johnson, Christopher] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Kim, JK (reprint author), Ulsan Natl Inst Sci & Technol, Dept Energy & Chem Engn, Ulsan 689798, South Korea. EM jpcho@unist.ac.kr; ykim@unist.ac.kr RI Kim, Youngsik/B-3570-2014; Cho, Jaephil/E-4265-2010 FU Creativity and Innovation Project Fund of Ulsan National Institute of Science and Technology (UNIST) [1,140009,01]; Basic Science Research Program through the National Research Foundation of Korea (NRF) - Ministry of Education [NRF-2014R1A1A2A16053515]; C-ITRC (Convergence Information Technology Research Center) support program [NIPA-2013-H0301-13-1009]; Department of Energy [DE-AC02-06CH11357] FX This work was supported by the Creativity and Innovation Project Fund (1,140009,01) of Ulsan National Institute of Science and Technology (UNIST) and the Basic Science Research Program through the National Research Foundation of Korea (NRF) funded by the Ministry of Education (NRF-2014R1A1A2A16053515). A part of this work was also supported by the C-ITRC (Convergence Information Technology Research Center) support program (NIPA-2013-H0301-13-1009) supervised by the NIPA (National IT Industry Promotion Agency) through the Ministry of Science, ICT and Future Planning, Korea. Funding for the Argonne National Laboratory is from the Department of Energy (Contract DE-AC02-06CH11357) and is gratefully acknowledged. NR 17 TC 9 Z9 9 U1 7 U2 44 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 2196-0216 J9 CHEMELECTROCHEM JI ChemElectroChem PD MAR 11 PY 2015 VL 2 IS 3 BP 328 EP 332 DI 10.1002/celc.201402344 PG 5 WC Electrochemistry SC Electrochemistry GA CD7UD UT WOS:000351298300003 ER PT J AU Shi, FF Ross, PN Zhao, H Liu, G Somorjai, GA Komvopoulos, K AF Shi, Feifei Ross, Philip N. Zhao, Hui Liu, Gao Somorjai, Gabor A. Komvopoulos, Kyriakos TI A Catalytic Path for Electrolyte Reduction in Lithium-Ion Cells Revealed by in Situ Attenuated Total Reflection-Fourier Transform Infrared Spectroscopy SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID NOBLE-METAL ELECTRODES; SURFACE-FILM FORMATION; SALT-SOLUTIONS; ELECTROCHEMICAL REDUCTION; CARBONATE ELECTROLYTES; ETHYLENE CARBONATE; TIN ELECTRODES; LI; BATTERIES; BEHAVIOR AB Although controlling the interfacial chemistry of electrodes in Li-ion batteries (LIBs) is crucial for maintaining the reversibility) electrolyte decomposition has not been,fully understood,. In this study, electrolyte decomposition on model electrode surfaces (Au and Sn) was investigated by in situ attenuated total reflection Fourier transform infrared (ATR-FTIR) spectroscopy. Simultaneously obtained ATR-FTIR. spectra and cyclic voltammetry. measurements show that lithium ethylene dicarbonate and lithium propionate form on the Au electrode at 0.6 V, whereas diethyl 2,5-dioxaheiane dicarboxylate and lithium propionate form on the Sn electrode surface at 1.25 V. A noncatalytic reduction path on the An surface and a catalytic reduction path on the Sn surface are introduced to explain the surface dependence of the overpotential and product selectivity. This represents' a new concept for explaining electrolyte reactions on the anode of LIBs. The present investigation shows that catalysis plays a, dominant role in the electrolyte decomposition process and. has important implications in electrode surface :modification, and electrolyte recipe selection, which are critical factors for enhancing the efficiency, durability, and reliability of LIBs. C1 [Shi, Feifei; Komvopoulos, Kyriakos] Univ Calif Berkeley, Dept Mech Engn, Berkeley, CA 94720 USA. [Somorjai, Gabor A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Shi, Feifei; Ross, Philip N.; Somorjai, Gabor A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Zhao, Hui; Liu, Gao] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. RP Somorjai, GA (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM somorjai@berkeley.edu; kyriakos@me.berkeley.edu FU Office of Freedom CAR and Vehicle Technologies of the U.S. Department of Energy [DE-AC02 O5CH1123]; UCB-KAUST Academic Excellence Alliance (AEA) Program; Office of Basic Energy Sciences, Materials Science and Engineering Division of the U.S, Department of Energy FX This work was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Freedom CAR and Vehicle Technologies of the U.S. Department of Energy under Contract No. DE-AC02 O5CH1123. The last author (K.K.) also acknowledges the funding provided for this work by the UCB-KAUST Academic Excellence Alliance (AEA) Program. The IR instrumentation was purchased with funding from the Director, Office of Basic Energy Sciences, Materials Science and Engineering Division of the U.S, Department of Energy. NR 35 TC 9 Z9 9 U1 10 U2 81 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAR 11 PY 2015 VL 137 IS 9 BP 3181 EP 3184 DI 10.1021/ja5128456 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA CD6GI UT WOS:000351187200008 PM 25689135 ER PT J AU Nelson, HM Williams, BD Miro, J Toste, FD AF Nelson, Hosea M. Williams, Brett D. Miro, Javier Toste, F. Dean TI Enantioselective 1,1-Arylborylation of Alkenes: Merging Chiral Anion Phase Transfer with Pd Catalysis SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID ASYMMETRIC HYDROBORATION; PALLADIUM CATALYSIS; GRIGNARD-REAGENTS; FLUORINATION; ESTERS; ACIDS; CONSTRUCTION; ALLYLATION; ALDEHYDES; ALCOHOLS AB A palladium-catalyzed three-Component coupling of alpha-olefins, aryldiazonium salts, and bis-(pinacolato)diboron affords direct access to chiral benzylic boronic esters. This process is rendered highly enantioselective using an unprecedented example of cooperative chiral anion phase transfer and tiansition-metal catalysis. C1 [Toste, F. Dean] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Toste, FD (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM fdtoste@berkeley.edu FU NIGMS [R01 GM104534]; UNCF; Merck; University of Valencia FX We gratefully acknowledge the NIGMS (R01 GM104534) for financial support. We acknowledge Prof. Matthew Sigman for useful discussions and experimental advice. H.M.N. also acknowledges the UNCF and Merck for generous funding. J.M. thanks the University of Valencia for a predoctoral fellowship. NR 41 TC 25 Z9 25 U1 6 U2 53 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAR 11 PY 2015 VL 137 IS 9 BP 3213 EP 3216 DI 10.1021/jacs.5b00344 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA CD6GI UT WOS:000351187200016 PM 25723255 ER PT J AU Rajput, NN Qu, XH Sa, N Burrell, AK Persson, KA AF Rajput, Nav Nidhi Qu, Xiaohui Sa, Niya Burrell, Anthony K. Persson, Kristin A. TI The Coupling between Stability and Ion Pair Formation in Magnesium Electrolytes from First-Principles Quantum Mechanics and Classical Molecular Dynamics SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID ORGANIC-SOLVENTS; ENERGY-STORAGE; ELECTROCHEMICAL WINDOWS; POLYMER ELECTROLYTES; LITHIUM BATTERIES; FORCE-FIELD; AB-INITIO; SIMULATIONS; SOLVATION; COMPLEX AB In this work we uncover a novel effect between concentration dependent ion pair formation and anion stability at reducing potentials, e.g., at the metal anode. Through comprehensive calculations using both first-principles as well as well-benchmarked classical molecular dynamics over a matrix of electrolytes, covering solvents and salt anions with a broad range in chemistry, we elucidate systematic correlations between molecular level interactions and composite electrolyte properties, such as electrochemical stability, solvation structure, and dynamics. We find that Mg electrolytes are highly prone to ion pair formation, even at modest concentrations, for a wide range of solvents with different dielectric constants, which have implications for dynamics as well as charge transfer. Specifically, we observe that, at Mg metal potentials, the ion pair undergoes partial reduction at the Mg cation center (Mg2+ -> Mg+), which competes with the charge transfer mechanism and can activate the anion to render it susceptible to decomposition. Specifically, TFSI exhibits a significant bond weakening while paired with the transient, partially reduced Mg+. In contrast, BH4 and BF4 are shown to be chemically stable in a reduced ion pair configuration. Furthermore, we observe that higher order glymes as well as DMSO improve the solubility of Mg salts, but only the longer glyme chains reduce the dynamics of the ions in solution. This information provides critical design metrics for future electrolytes as it elucidates a close connection between bulk solvation and cathodic stability as well as the dynamics of the salt. C1 [Rajput, Nav Nidhi; Qu, Xiaohui; Persson, Kristin A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Sa, Niya; Burrell, Anthony K.] Argonne Natl Lab, Chem Sci & Engn, Lemont, IL 60439 USA. RP Persson, KA (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. EM kapersson@lbl.gov RI SA, NIYA/E-8521-2017 FU Joint Center for Energy Storage Research (JCESR), an Energy Innovation Hub - U.S. Department of Energy [DE-AC02-06CH11357]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; Materials Project (BES DOE) [EDCBEE] FX This work was supported as part of the Joint Center for Energy Storage Research (JCESR), an Energy Innovation Hub funded by the U.S. Department of Energy, under Contract No. DE-AC02-06CH11357. High performance computational resources for this research were provided by the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The Materials Project (BES DOE Grant No. EDCBEE) is acknowledged for infrastructure and algorithmic support. NR 75 TC 36 Z9 36 U1 12 U2 144 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAR 11 PY 2015 VL 137 IS 9 BP 3411 EP 3420 DI 10.1021/jacs.5b01004 PG 10 WC Chemistry, Multidisciplinary SC Chemistry GA CD6GI UT WOS:000351187200044 PM 25668289 ER PT J AU Wilson, RB Apgar, BA Hsieh, WP Martin, LW Cahill, DG AF Wilson, R. B. Apgar, Brent A. Hsieh, Wen-Pin Martin, Lane W. Cahill, David G. TI Thermal conductance of strongly bonded metal-oxide interfaces SO PHYSICAL REVIEW B LA English DT Article ID TIME-DOMAIN THERMOREFLECTANCE; 300 DEGREES K; ELASTIC-CONSTANTS; LATTICE-DYNAMICS; BOUNDARY RESISTANCE; MAGNESIUM-OXIDE; HEAT-TRANSPORT; CONDUCTIVITY; PRESSURE; ALUMINUM AB We report the results of time-domain thermoreflectance (TDTR) measurements of two strongly bonded metal-oxide systems with unusually large thermal conductances. We find that TDTR data for the epitaxial SrRuO3/SrTiO3 interface is consistent with an interface conductance G > 0.8 GW m(-2) K-1. For an Al/MgO interface at a pressure of 60 GPa, we find G approximate to 1.1 GW m(-2) K-1. Both are within 40% of the maximum possible conductance for these systems, as predicted by simple theory. C1 [Wilson, R. B.; Apgar, Brent A.; Hsieh, Wen-Pin; Martin, Lane W.; Cahill, David G.] Univ Illinois, Dept Mat Sci & Engn, Urbana, IL 61801 USA. [Wilson, R. B.; Apgar, Brent A.; Hsieh, Wen-Pin; Martin, Lane W.; Cahill, David G.] Univ Illinois, Mat Res Lab, Urbana, IL 61801 USA. [Apgar, Brent A.; Martin, Lane W.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Apgar, Brent A.] Int Inst Carbon Neutral Energy Res, Nishi Ku, Fukuoka 8190395, Japan. [Hsieh, Wen-Pin] Acad Sinica, Inst Earth Sci, Taipei 11529, Taiwan. [Martin, Lane W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Wilson, RB (reprint author), Univ Illinois, Dept Mat Sci & Engn, 1304 W Green St, Urbana, IL 61801 USA. EM wilson81@illinois.edu RI Martin, Lane/H-2409-2011; Hsieh, Wen-Pin/M-8479-2014 OI Martin, Lane/0000-0003-1889-2513; FU US Department of Energy, Office of Basic Energy Sciences [DE-FG02-07ER46459]; International Institute for Carbon-Neutral Energy Research (WPI-I2CNER) - Japanese Ministry of Education, Culture, Sport, Science and Technology; Carnegie-DOE Alliance Center (CDAC) [DE-FC52-08NA28554]; Department of Defense FX Experimental work on epitaxial oxide interfaces and theoretical analysis of thermal conductance were supported by the US Department of Energy, Office of Basic Energy Sciences under Award Grant No. DE-FG02-07ER46459. B.A.A. and L.W.M. acknowledge funding support from the International Institute for Carbon-Neutral Energy Research (WPI-I2CNER), sponsored by the Japanese Ministry of Education, Culture, Sport, Science and Technology. W.-P.H. acknowledges support from the Carnegie-DOE Alliance Center (CDAC) through grant DE-FC52-08NA28554. Experiments were carried out in part in the Frederick Seitz Materials Research Laboratory Central Research Facilities, University of Illinois. R.B.W. thanks the Department of Defense for the NDSEG fellowship that supported him during this work and Gyung-Min Choi for his assistance with the optical calculations. NR 59 TC 7 Z9 7 U1 3 U2 25 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 11 PY 2015 VL 91 IS 11 AR 115414 DI 10.1103/PhysRevB.91.115414 PG 7 WC Physics, Condensed Matter SC Physics GA CD3DR UT WOS:000350958500005 ER PT J AU Szymanska, P Martin, KR MacKeigan, JP Hlavacek, WS Lipniacki, T AF Szymanska, Paulina Martin, Katie R. MacKeigan, Jeffrey P. Hlavacek, William S. Lipniacki, Tomasz TI Computational Analysis of an Autophagy/Translation Switch Based on Mutual Inhibition of MTORC1 and ULK1 SO PLOS ONE LA English DT Article ID ACTIVATED PROTEIN-KINASE; EUKARYOTIC GENE-EXPRESSION; DEPENDENT PHOSPHORYLATION; MAMMALIAN TARGET; MAINTAINS ENERGY; BINDING PARTNER; CELL-GROWTH; AMINO-ACIDS; S6 KINASE; AUTOPHAGY AB We constructed a mechanistic, computational model for regulation of (macro) autophagy and protein synthesis (at the level of translation). The model was formulated to study the system-level consequences of interactions among the following proteins: two key components of MTOR complex 1 (MTORC1), namely the protein kinase MTOR (mechanistic target of rapamycin) and the scaffold protein RPTOR; the autophagy-initiating protein kinase ULK1; and the multimeric energy-sensing AMP-activated protein kinase (AMPK). Inputs of the model include intrinsic AMPK kinase activity, which is taken as an adjustable surrogate parameter for cellular energy level or AMP: ATP ratio, and rapamycin dose, which controls MTORC1 activity. Outputs of the model include the phosphorylation level of the translational repressor EIF4EBP1, a substrate of MTORC1, and the phosphorylation level of AMBRA1 (activating molecule in BECN1-regulated autophagy), a substrate of ULK1 critical for autophagosome formation. The model incorporates reciprocal regulation of mTORC1 and ULK1 by AMPK, mutual inhibition of MTORC1 and ULK1, and ULK1-mediated negative feedback regulation of AMPK. Through analysis of the model, we find that these processes may be responsible, depending on conditions, for graded responses to stress inputs, for bistable switching between autophagy and protein synthesis, or relaxation oscillations, comprising alternating periods of autophagy and protein synthesis. A sensitivity analysis indicates that the prediction of oscillatory behavior is robust to changes of the parameter values of the model. The model provides testable predictions about the behavior of the AMPK-MTORC1-ULK1 network, which plays a central role in maintaining cellular energy and nutrient homeostasis. C1 [Szymanska, Paulina] Univ Warsaw, Coll Inter, Fac Individual Studies Math & Nat Sci, Warsaw, Poland. [Martin, Katie R.; MacKeigan, Jeffrey P.] Van Andel Inst, Grand Rapids, MI USA. [Hlavacek, William S.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87544 USA. [Hlavacek, William S.] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. [Lipniacki, Tomasz] Inst Fundamental Technol Res, PL-00049 Warsaw, Poland. RP Hlavacek, WS (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87544 USA. EM wish@lanl.gov; tlipnia@ippt.pan.pl OI Lipniacki, Tomasz/0000-0002-3488-2561; Hlavacek, William/0000-0003-4383-8711 FU National Institutes of Health/National Institute of General Medical Science [P50GM085273]; US Department of Energy through the Los Alamos Center for Nonlinear Studies [DE-AC52-06NA25396]; Laboratory-directed Research and Development (LDRD) Program; National Science Center (Poland) [2011/03/B/NZ2/00281]; EU through the European Social Fund [UDA-POKL.04.01.01-00-072/09-00] FX WSH is supported by National Institutes of Health/National Institute of General Medical Science grant P50GM085273, (www.nih.gov/www.nigms.nih.gov) and US Department of Energy Contract DE-AC52-06NA25396 through the Los Alamos Center for Nonlinear Studies and the Laboratory-directed Research and Development (LDRD) Program, (www.energy.gov). TL is supported by National Science Center (Poland) Grant No. 2011/03/B/NZ2/00281, (www.ncn.gov.pl). PS is supported by EU through the European Social Fund, contract number UDA-POKL.04.01.01-00-072/09-00, (http://ec.europa.eu). The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 69 TC 4 Z9 4 U1 0 U2 8 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAR 11 PY 2015 VL 10 IS 3 AR e0116550 DI 10.1371/journal.pone.0116550 PG 34 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CD7MQ UT WOS:000351275000006 PM 25761126 ER PT J AU Bock, DC Tappero, RV Takeuchi, KJ Marschilok, AC Takeuchi, ES AF Bock, David C. Tappero, Ryan V. Takeuchi, Kenneth J. Marschilok, Amy C. Takeuchi, Esther S. TI Mapping the Anode Surface-Electrolyte Interphase: Investigating a Life Limiting Process of Lithium Primary Batteries SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE Silver vanadium oxide; silver vanadium phosphorus oxide; X-ray microfluorescence mapping; solid electrolyte interphase; lithium battery ID SILVER VANADIUM-OXIDE; IMPLANTABLE CARDIOVERTER-DEFIBRILLATORS; RAY-ABSORPTION SPECTROSCOPY; ION BATTERIES; ELECTROCHEMICAL PROPERTIES; DISSOLUTION KINETICS; POSITIVE ELECTRODE; CATHODE MATERIALS; CRYSTAL-STRUCTURE; CAPACITY LOSSES AB Cathode solubility in batteries can lead to decreased and unpredictable long-term battery behavior due to transition metal deposition on the negative electrode such that it no longer supports high current. Analysis of negative electrodes from cells containing vanadium oxide or phosphorus oxide based cathode systems retrieved after long-term testing was conducted. This report demonstrates the use of synchrotron based X-ray microfluorescence (XR mu F) to map negative battery electrodes in conjunction with microbeam X-ray absorption spectroscopy (mu XAS) to determine the oxidation states of the metal centers resident in the solid electrolyte interphase (SEI) and at the electrode surface. Based on the empirical findings, a conceptual model for the location of metal ions in the SEI and their role in impacting lithium ion mobility at the electrode surfaces is proposed. C1 [Bock, David C.; Takeuchi, Kenneth J.; Marschilok, Amy C.; Takeuchi, Esther S.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Tappero, Ryan V.; Takeuchi, Esther S.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Takeuchi, Kenneth J.; Marschilok, Amy C.; Takeuchi, Esther S.] SUNY Stony Brook, Dept Mat Sci & Engn, Stony Brook, NY 11794 USA. RP Takeuchi, KJ (reprint author), SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. EM kenneth.takeuchi.1@stonybrook.edu; amy.marschilok@stonybrook.edu; esther.takeuchi@stonybrook.edu FU National Institutes of Health from the National Heart, Lung, and Blood Institute [1R01HL093044-01A1]; DOE- Geosciences [DE-FG02-92ER14244]; DOE [DE-AC02-98CH10886]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX The synthesis, characterization, and pulse discharge studies were supported by the National Institutes of Health under Grant 1R01HL093044-01A1 from the National Heart, Lung, and Blood Institute. Mechanistic investigation of the material via XRF was supported by the Department of Energy, Office of Basic Energy Sciences. Portions of this work were performed at Beamline X27A, National Synchrotron Light Source (NSLS), Brookhaven National Laboratory (BNL). X27A is supported in part by DOE- Geosciences (DE-FG02-92ER14244 to The University of Chicago-CARS). Use of NSLS I was supported by the DOE under Contract No. DE-AC02-98CH10886. The authors acknowledge Jurgen Thieme and Paul Northrup for helpful discussions relevant to the XRF experiments. Development of the experimental methodology for XRF measurement was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. NR 56 TC 5 Z9 5 U1 7 U2 78 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD MAR 11 PY 2015 VL 7 IS 9 BP 5429 EP 5437 DI 10.1021/am509066n PG 9 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA CC8JN UT WOS:000350614600049 PM 25690846 ER PT J AU Bai, Y Wang, Z Wu, C Xu, R Wu, F Liu, YC Li, H Li, Y Lu, J Amine, K AF Bai, Ying Wang, Zhen Wu, Chuan Xu, Rui Wu, Feng Liu, Yuanchang Li, Hui Li, Yu Lu, Jun Amine, Khalil TI Hard Carbon Originated from Polyvinyl Chloride Nanofibers As High-Performance Anode Material for Na-Ion Battery SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE Na-ion battery; hard carbon; polyvinyl chloride nanofiber; electrospinning ID ELECTROCHEMICAL INSERTION; HIGH-CAPACITY; ENERGY-STORAGE; SODIUM; ELECTRODES; FIBERS; CHALLENGES; NANOWIRES AB Two types of hard carbon materials were synthesized through direct pyrolysis of commercial polyvinyl chloride (PVC) particles and pyrolysis of PVC nanofibers at 600-800 degrees C, respectively, where the nanofibers were prepared by an electrospinning PVC precursors method. These as-prepared hard carbon samples were used as anode materials for Na-ion batteries. The hard carbon obtained from PVC nanofibers achieved a high reversible capacity of 271 mAh/g and an initial Coulombic efficiency of 69.9%, which were much superior to the one from commercial PVC, namely, a reversible capacity of 206 mAh/g and an initial Coulombic efficiency of 60.9%. In addition, the hard carbon originated from the PVC nanofibers exhibited good cycling stability and rate performance: the initial discharge capacities were 389, 228, 194, 178, 147 mAh/g at the current density of 12, 24, 60, 120, and 240 mA/g, respectively, retaining 211 mAh/g after 150 cycles. Such excellent cycle performance, high reversible capacity, and good rate capability enabled this hard carbon to be a promising candidate as anode material for Na-ion battery application. C1 [Bai, Ying; Wang, Zhen; Wu, Chuan; Wu, Feng; Liu, Yuanchang; Li, Hui; Li, Yu] Beijing Inst Technol, Sch Chem Engn & Environm, Beijing Key Lab Environm Sci & Engn, Beijing 100081, Peoples R China. [Xu, Rui; Lu, Jun; Amine, Khalil] Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA. RP Wu, F (reprint author), Beijing Inst Technol, Sch Chem Engn & Environm, Beijing Key Lab Environm Sci & Engn, Beijing 100081, Peoples R China. EM wufeng863@bit.edu.cn; junlu@anl.gov; amine@anl.gov RI wu, chuan/A-1447-2009 FU National Basic Research Program of China [2015CB251100]; Program for New Century Excellent Talents in University [NCET-13-0033]; Beijing Higher Institution Engineering Research Center of Power Battery and Chemical Energy Materials; U.S. Department of Energy by UChicago Argonne, LLC [DE-AC02-06CH11357]; State Scholarship Fund of the China Scholarship Council [201406035025] FX This work is supported by National Basic Research Program of China (Grant No. 2015CB251100), Program for New Century Excellent Talents in University (Grant NCET-13-0033), and Beijing Higher Institution Engineering Research Center of Power Battery and Chemical Energy Materials. Argonne National Laboratory is operated for the U.S. Department of Energy by UChicago Argonne, LLC, under contract DE-AC02-06CH11357. Y.B. acknowledges the support from the State Scholarship Fund (201406035025) of the China Scholarship Council. NR 26 TC 48 Z9 48 U1 31 U2 170 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD MAR 11 PY 2015 VL 7 IS 9 BP 5598 EP 5604 DI 10.1021/acsami.5b00861 PG 7 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA CC8JN UT WOS:000350614600068 PM 25692826 ER PT J AU Draguta, S McDaniel, H Klimov, VI AF Draguta, Sergiu McDaniel, Hunter Klimov, Victor I. TI Tuning Carrier Mobilities and Polarity of Charge Transport in Films of CuInSexS2-x Quantum Dots SO ADVANCED MATERIALS LA English DT Article ID FIELD-EFFECT TRANSISTORS; NANOCRYSTAL SOLAR-CELLS; ELECTRICAL-PROPERTIES; PHOTOVOLTAIC DEVICES; THIN-FILMS; PBSE; PERFORMANCE; SOLIDS; SEMICONDUCTOR; TEMPERATURE C1 [Draguta, Sergiu; McDaniel, Hunter; Klimov, Victor I.] Los Alamos Natl Lab, Ctr Adv Solar Photophys, Los Alamos, NM 87545 USA. RP McDaniel, H (reprint author), Los Alamos Natl Lab, Ctr Adv Solar Photophys, POB 1663, Los Alamos, NM 87545 USA. EM hunter@ubiqd.com; klimov@lanl.gov OI Klimov, Victor/0000-0003-1158-3179 FU Center for Advanced Solar Photophysics (CASP), an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences FX This material was based upon work supported by the Center for Advanced Solar Photophysics (CASP), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. NR 47 TC 9 Z9 9 U1 10 U2 62 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD MAR 11 PY 2015 VL 27 IS 10 BP 1701 EP + DI 10.1002/adma.201404878 PG 6 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA CD0II UT WOS:000350754100008 PM 25613726 ER PT J AU Herklotz, A Dorr, K AF Herklotz, Andreas Doerr, Kathrin TI Characterization of tetragonal phases of SrRuO3 under epitaxial strain by density functional theory SO EUROPEAN PHYSICAL JOURNAL B LA English DT Article ID THIN-FILMS; PEROVSKITES; TRANSITION AB Using density functional theory calculations we study the effect of strain on the magnetic and structural properties of tetragonal SrRuO3. All four different oxygen octahedra rotation patterns that are in agreement with tetragonal symmetry are considered and compared with the bulk-like orthorhombic structure. We find that among the tetragonal structures the phase with I4/mcm symmetry is energetically most favorable. This structure is also lower in energy than the orthorhombic phase for compressive and tensile strain larger than -2.1% and +3.8%, respectively. The stability of the magnetic moment is found to be greatly dependent on the octahedra rotation pattern. The magnetic moment of the zero or one-tilt systems is quenched under tensile strain, while ferromagnetic order is preserved in the two or three-tilt systems. C1 [Herklotz, Andreas] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Doerr, Kathrin] Univ Halle Wittenberg, Inst Phys, D-06108 Halle, Germany. RP Herklotz, A (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. EM herklotza@gmail.com FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Science and Engineering Division; DFG [SFB 762] FX This work was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Science and Engineering Division and the DFG SFB 762. NR 32 TC 1 Z9 1 U1 5 U2 25 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6028 EI 1434-6036 J9 EUR PHYS J B JI Eur. Phys. J. B PD MAR 11 PY 2015 VL 88 IS 3 AR 60 DI 10.1140/epjb/e2015-50843-9 PG 5 WC Physics, Condensed Matter SC Physics GA CD5QC UT WOS:000351141900004 ER PT J AU Aceves, AB Shtyrina, OV Rubenchik, AM Fedoruk, MP Turitsyn, SK AF Aceves, Alejandro B. Shtyrina, Olga V. Rubenchik, Alexander M. Fedoruk, Mikhail P. Turitsyn, Sergei K. TI Spatiotemporal optical bullets in two-dimensional fiber arrays and their stability SO PHYSICAL REVIEW A LA English DT Article ID LIGHT BULLETS; SOLITONS; COLLAPSE; SYSTEMS; LASERS AB Long-lived light bullets fully localized in both space and time can be generated in novel photonic media such as multicore optical fiber or waveguide arrays. In this paper we present detailed theoretical analysis on the existence and stability of the discrete-continuous light bullets using a very generic model that occurs in a number of applications. C1 [Aceves, Alejandro B.] So Methodist Univ, Dept Math, Dallas, TX 75275 USA. [Shtyrina, Olga V.; Fedoruk, Mikhail P.; Turitsyn, Sergei K.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Shtyrina, Olga V.; Fedoruk, Mikhail P.] Inst Computat Technol, Novosibirsk 630090, Russia. [Rubenchik, Alexander M.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Turitsyn, Sergei K.] Aston Univ, Aston Inst Photon Technol, Birmingham B4 7ET, W Midlands, England. RP Aceves, AB (reprint author), So Methodist Univ, Dept Math, Dallas, TX 75275 USA. OI shtyrina, olya/0000-0002-0433-1427 FU Ministry of Education and Science of the Russian Federation [14.B25.31.0003]; Russian Science Foundation [14-21-00110]; Air Force EOARD [FA9550-14-1-0305]; US Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Army Research Department under MURI [W911NF-11-0297] FX We acknowledge support from a grant from the Ministry of Education and Science of the Russian Federation (Agreement No. 14.B25.31.0003), the Russian Science Foundation (Grant No. 14-21-00110) (the work of O.V.S. and M.P.F.), and the Air Force EOARD (Grant No. FA9550-14-1-0305). This work was partially performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. A.B.A.'s work was supported by the Army Research Department under MURI Grant No. W911NF-11-0297. NR 33 TC 3 Z9 3 U1 1 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1050-2947 EI 1094-1622 J9 PHYS REV A JI Phys. Rev. A PD MAR 11 PY 2015 VL 91 IS 3 AR 033810 DI 10.1103/PhysRevA.91.033810 PG 6 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA CD3CU UT WOS:000350956200006 ER PT J AU Iacocca, E Durrenfeld, P Heinonen, O Akerman, J Dumas, RK AF Iacocca, Ezio Durrenfeld, Philipp Heinonen, Olle Akerman, Johan Dumas, Randy K. TI Mode-coupling mechanisms in nanocontact spin-torque oscillators SO PHYSICAL REVIEW B LA English DT Article ID NANO-OSCILLATORS; BUILDING-BLOCKS; DRIVEN; WAVES AB Spin-torque oscillators (STOs) are devices that allow for the excitation of a variety of magnetodynamical modes at the nanoscale. Depending on both external conditions and intrinsic magnetic properties, STOs can exhibit regimes of mode hopping and even mode coexistence. Whereas mode hopping has been extensively studied in STOs patterned as nanopillars, coexistence has been only recently observed for localized modes in nanocontact STOs (NC-STOs), where the current is confined to flow through a NC fabricated on an extended pseudo spin valve. By means of electrical characterization and a multimode STO theory, we investigate the physical origin of the mode-couplingmechanisms favoring coexistence. Two couplingmechanisms are identified: (i) magnon-mediated scattering and (ii) intermode interactions. These mechanisms can be physically disentangled by fabricating devices where the NCs have an elliptical cross section. The generation power and linewidth from such devices are found to be in good qualitative agreement with the theoretical predictions, as well as provide evidence of the dominant mode-coupling mechanisms. C1 [Iacocca, Ezio; Durrenfeld, Philipp; Akerman, Johan; Dumas, Randy K.] Univ Gothenburg, Dept Phys, S-41296 Gothenburg, Sweden. [Iacocca, Ezio; Akerman, Johan; Dumas, Randy K.] NanOsc AB, S-16440 Kista, Sweden. [Heinonen, Olle] Argonne Natl Lab, Div Mat Sci, Lemont, IL 60439 USA. [Heinonen, Olle] Nrothwestern Argonne Inst Sci & Engn, Evanston, IL 60208 USA. [Akerman, Johan] Royal Inst Technol, Sch ICT, Mat Phys, S-16440 Kista, Sweden. RP Iacocca, E (reprint author), Univ Gothenburg, Dept Phys, S-41296 Gothenburg, Sweden. RI Dumas, Randy/E-3077-2010; Akerman, Johan/B-5726-2008; OI Dumas, Randy/0000-0001-5505-2172; Akerman, Johan/0000-0002-3513-6608; Heinonen, Olle/0000-0002-3618-6092; Iacocca, Ezio/0000-0002-8870-5106; Durrenfeld, Philipp/0000-0002-6219-4862 FU European Commission [317950]; Department of Energy Office of Science, Materials Sciences and Engineering Division; Knut and Alice Wallenberg Foundation; Swedish Foundation for Strategic Research (S.S.F.); Swedish Research Council (V.R.) FX This work was supported by the European Commission FP7-ICT-2011, Contract No. 317950 "MOSAIC." The work by O.H. was funded by the Department of Energy Office of Science, Materials Sciences and Engineering Division. Support from the Swedish Research Council (V.R.), the Swedish Foundation for Strategic Research (S.S.F.), and the Knut and Alice Wallenberg Foundation is gratefully acknowledged. NR 37 TC 6 Z9 6 U1 3 U2 24 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 11 PY 2015 VL 91 IS 10 AR 104405 DI 10.1103/PhysRevB.91.104405 PG 7 WC Physics, Condensed Matter SC Physics GA CD3DK UT WOS:000350957800001 ER PT J AU Jamer, ME Assaf, BA Sterbinsky, GE Arena, D Lewis, LH Saul, AA Radtke, G Heiman, D AF Jamer, M. E. Assaf, B. A. Sterbinsky, G. E. Arena, D. Lewis, L. H. Saul, A. A. Radtke, G. Heiman, D. TI Antiferromagnetic phase of the gapless semiconductor V3Al SO PHYSICAL REVIEW B LA English DT Article AB Discovering new antiferromagnetic (AF) compounds is at the forefront of developing future spintronic devices without fringing magnetic fields. TheAF gapless semiconducting D0(3) phase of V-3 Al was successfully synthesized via arc-melting and annealing. The AF properties were established through synchrotron measurements of the atom-specific magnetic moments, where the magnetic dichroism reveals large and oppositely oriented moments on individual V atoms. Density functional theory calculations confirmed the stability of a type G antiferromagnetism involving only two-thirds of the V atoms, while the remaining V atoms are nonmagnetic. Magnetization, x-ray diffraction, and transport measurements also support the antiferromagnetism. This archetypal gapless semiconductor may be considered as a cornerstone for future spintronic devices containing AF elements. C1 [Jamer, M. E.; Assaf, B. A.; Heiman, D.] Northeastern Univ, Dept Phys, Boston, MA 02115 USA. [Sterbinsky, G. E.; Arena, D.] Brookhaven Natl Lab, Photon Sci Directorate, Upton, NY 11973 USA. [Lewis, L. H.] Northeastern Univ, Dept Chem Engn, Boston, MA 02115 USA. [Saul, A. A.] Aix Marseille Univ, CINaM, CNRS, UMR 7325, F-13288 Marseille 9, France. [Saul, A. A.] MIT, Dept Civil & Environm Engn, Cambridge, MA 02139 USA. [Radtke, G.] Univ Paris 06, Sorbonne Univ, IMPMC, Museum Natl Hist Nat, F-75005 Paris, France. RP Jamer, ME (reprint author), Northeastern Univ, Dept Phys, Boston, MA 02115 USA. RI Saul, Andres/C-1282-2012; OI Saul, Andres/0000-0003-0540-703X; Jamer, Michelle/0000-0001-5316-8817 FU National Science Foundation [DMR-0907007, ECCS-1402738]; U.S. Department of Energy; Office of Science, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX We thank I. McDonald for his assistance with VSM measurements and thank F. Jimenez-Villacorta, T. Devakul, and A. Feiguin for helpful discussions. The paper was supported by the National Science Foundation Grants No. DMR-0907007 and No. ECCS-1402738. This paper was granted access to the High Performance Computing (HPC) resources of Institut du Developpement et des Ressources en Informatique Scientifique (IDRIS) under the allocations 2014-100384 made by Grand Equipement National de Calcul Intensif (GENCI). Use of the NSLS, Brookhaven National Laboratory, was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. We thank J. Bai at beamline X14A at NSLS. M.E.J. was supported by the International Centre for Diffraction Data's Ludo Frevel Scholarship. NR 28 TC 9 Z9 9 U1 2 U2 22 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 11 PY 2015 VL 91 IS 9 AR 094409 DI 10.1103/PhysRevB.91.094409 PG 5 WC Physics, Condensed Matter SC Physics GA CD3DD UT WOS:000350957100003 ER PT J AU Radin, MD Ogitsu, T Biener, J Otani, M Wood, BC AF Radin, Maxwell D. Ogitsu, Tadashi Biener, Juergen Otani, Minoru Wood, Brandon C. TI Capacitive charge storage at an electrified interface investigated via direct first-principles simulations SO PHYSICAL REVIEW B LA English DT Article ID GENERALIZED GRADIENT APPROXIMATION; QUANTUM CAPACITANCE; SUPERCAPACITOR ELECTRODES; CARBON MATERIALS; ENERGY-STORAGE; GRAPHENE; LAYER; ULTRACAPACITORS; GRAPHITE; DENSITY AB Understanding the impact of interfacial electric fields on electronic structure is crucial to improving the performance of materials in applications based on charged interfaces. Supercapacitors store energy directly in the strong interfacial field between a solid electrode and a liquid electrolyte; however, the complex interplay between the two is often poorly understood, particularly for emerging low-dimensional electrode materials that possess unconventional electronic structure. Typical descriptions tend to neglect the specific electrode-electrolyte interaction, approximating the intrinsic "quantum capacitance" of the electrode in terms of a fixed electronic density of states. Instead, we introduce a more accurate first-principles approach for directly simulating charge storage in model capacitors using the effective screening medium method, which implicitly accounts for the presence of the interfacial electric field. Applying this approach to graphene supercapacitor electrodes, we find that results differ significantly from the predictions of fixed-band models, leading to improved consistency with experimentally reported capacitive behavior. The differences are traced to two key factors: the inhomogeneous distribution of stored charge due to poor electronic screening and interfacial contributions from the specific interaction with the electrolyte. Our results are used to revise the conventional definition of quantum capacitance and to provide general strategies for improving electrochemical charge storage, particularly in graphene and similar low-dimensional materials. C1 [Radin, Maxwell D.] Univ Michigan, Dept Phys, Ann Arbor, MI 48105 USA. [Ogitsu, Tadashi; Biener, Juergen; Wood, Brandon C.] Lawrence Livermore Natl Lab, Div Sci Mat, Livermore, CA 94550 USA. [Otani, Minoru] Natl Inst Adv Ind Sci & Technol, Tsukuba, Ibaraki, Japan. RP Radin, MD (reprint author), Univ Calif Santa Barbara, Dept Mat, Santa Barbara, CA 93106 USA. EM brandonwood@llnl.gov FU US Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; LLNL Laboratory Directed Research and Development Program [12-ERD-035] FX This work was performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. Funding was provided by LLNL Laboratory Directed Research and Development Program Grant No. 12-ERD-035, with computing support from the LLNL Institutional Computing Grand Challenge Program. The authors acknowledge helpful discussions with M. Merrill and J. R. I. Lee. NR 44 TC 4 Z9 4 U1 8 U2 47 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAR 11 PY 2015 VL 91 IS 12 AR 125415 DI 10.1103/PhysRevB.91.125415 PG 7 WC Physics, Condensed Matter SC Physics GA CD3EG UT WOS:000350960100006 ER PT J AU Bramante, J Fox, PJ Martin, A Ostdiek, B Plehn, T Schell, T Takeuchi, M AF Bramante, Joseph Fox, Patrick J. Martin, Adam Ostdiek, Bryan Plehn, Tilman Schell, Torben Takeuchi, Michihisa TI Relic neutralino surface at a 100 TeV collider SO PHYSICAL REVIEW D LA English DT Article ID GAUGINO-PAIR PRODUCTION; DARK-MATTER; HADRON COLLIDERS; STAU COANNIHILATION; SPLIT SUPERSYMMETRY; STANDARD MODEL; MASS; PARTICLE; ABUNDANCE; PHYSICS AB We map the parameter space for minimal supersymmetric Standard Model neutralino dark matter which freezes out to the observed relic abundance, in the limit that all superpartners except the neutralinos and charginos are decoupled. In this space of relic neutralinos, we show the dominant dark matter annihilation modes, the mass splittings among the electroweakinos, direct detection rates, and collider cross sections. The mass difference between the dark matter and the next-to-lightest neutral and charged states is typically much less than electroweak gauge boson masses. With these small mass differences, the relic neutralino surface is accessible to a future 100 TeV hadron collider, which can discover interneutralino mass splittings down to 1 GeV and thermal relic dark matter neutralino masses up to 1.5 TeV with a few inverse attobarns of luminosity. This coverage is a direct consequence of the increased collider energy: in the Standard Model events with missing transverse momentum in the TeV range have mostly hard electroweak radiation, distinct from the soft radiation shed in compressed electroweakino decays. We exploit this kinematic feature in final states including photons and leptons, tailored to the 100 TeV collider environment. C1 [Bramante, Joseph; Martin, Adam; Ostdiek, Bryan] Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. [Fox, Patrick J.] Fermilab Natl Accelerator Lab, Dept Theoret Phys, Batavia, IL 60510 USA. [Plehn, Tilman; Schell, Torben] Heidelberg Univ, Inst Theoret Phys, D-69115 Heidelberg, Germany. [Takeuchi, Michihisa] Univ Tokyo, Kavli IPMU WPI, Kashiwa, Chiba, Japan. RP Bramante, J (reprint author), Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. OI Ostdiek, Bryan/0000-0002-0376-6461 FU IMPRS for Precision Tests of Fundamental Symmetries; National Science Foundation [PHY-1417118]; Notre Dame Center for Research Computing; World Premier International Research Center Initiative (WPI), MEXT, Japan; U.S. Department of Energy [DE-AC02-07CH11359] FX We would like to thank Vera Gluscevic, Rafael Lang, Annika Peter, and Pedro Schwaller for the discussions. J. B. is grateful to the CERN theory group for their hospitality while this paper was finalized. T. P. would like to thank the Fermilab Theory Group, where this project once started. T. S. acknowledges support from the IMPRS for Precision Tests of Fundamental Symmetries. The work of A. M. was partially supported by the National Science Foundation under Grant No. PHY-1417118. This research was supported in part by the Notre Dame Center for Research Computing with computing resources. This work was partially supported by World Premier International Research Center Initiative (WPI), MEXT, Japan. Fermilab is operated by Fermi Research Alliance, LLC under Contract No. DE-AC02-07CH11359 with the U.S. Department of Energy. NR 142 TC 27 Z9 27 U1 1 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 11 PY 2015 VL 91 IS 5 AR 054015 DI 10.1103/PhysRevD.91.054015 PG 17 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CD3GD UT WOS:000350965400004 ER PT J AU Cahill-Rowley, M Cotta, R Drlica-Wagner, A Funk, S Hewett, JL Ismail, A Rizzo, TG Wood, M AF Cahill-Rowley, M. Cotta, R. Drlica-Wagner, A. Funk, S. Hewett, J. L. Ismail, A. Rizzo, T. G. Wood, M. TI Complementarity of dark matter searches in the phenomenological MSSM SO PHYSICAL REVIEW D LA English DT Article ID CHERENKOV TELESCOPE ARRAY; PARTICLE; LHC; NEUTRALINO; CAPTURE; PROGRAM; DESIGN; BOSON AB As is well known, the search for and eventual identification of dark matter in supersymmetry requires a simultaneous, multipronged approach with important roles played by the LHC as well as both direct and indirect dark matter detection experiments. We examine the capabilities of these approaches in the 19-parameter phenomenological MSSM which provides a general framework for complementarity studies of neutralino dark matter. We summarize the sensitivity of dark matter searches at the 7 and 8 (and eventually 14) TeV LHC, combined with those by Fermi, CTA, IceCube/DeepCore, COUPP, LZ and XENON. The strengths and weaknesses of each of these techniques are examined and contrasted and their interdependent roles in covering the model parameter space are discussed in detail. We find that these approaches explore orthogonal territory and that advances in each are necessary to cover the supersymmetric weakly interacting massive particle parameter space. We also find that different experiments have widely varying sensitivities to the various dark matter annihilation mechanisms, some of which would be completely excluded by null results from these experiments. C1 [Cahill-Rowley, M.; Funk, S.; Hewett, J. L.; Rizzo, T. G.; Wood, M.] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Cotta, R.] Univ Calif Irvine, Irvine, CA 92697 USA. [Drlica-Wagner, A.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Ismail, A.] Argonne Natl Lab, Argonne, IL 60439 USA. [Ismail, A.] Univ Illinois, Chicago, IL 60607 USA. RP Cahill-Rowley, M (reprint author), SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. EM mrowley@slac.stanford.edu; cottar@uci.edu; kadrlica@fnal.gov; funk@slac.stanford.edu; hewett@slac.stanford.edu; aismail@anl.gov; rizzo@slac.stanford.edu; mdwood@slac.stanford.edu RI Funk, Stefan/B-7629-2015 OI Funk, Stefan/0000-0002-2012-0080 FU U.S. Department of Energy [DE-AC02-76SF00515, DE-AC02- 06CH11357, DE-FG02-12ER41811]; Department of Energy Office of Science Graduate Fellowship Program (DOE SCGF); ORISE-ORAU [DE-AC05-06OR23100]; National Science Foundation [PHY-0970173] FX The authors thank A. Barr, J. Buckley, D. Cote, J. Feng, K. Matchev, G. Redlinger, and T. Tait for useful discussions. This work was supported by the U.S. Department of Energy, Awards No. DE-AC02-76SF00515, No. DE-AC02- 06CH11357, and No. DE-FG02-12ER41811, and the Department of Energy Office of Science Graduate Fellowship Program (DOE SCGF), made possible in part by the American Recovery and Reinvestment Act of 2009, administered by ORISE-ORAU under Grant No. DE-AC05-06OR23100, and the National Science Foundation under Grant No. PHY-0970173. NR 54 TC 15 Z9 15 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 11 PY 2015 VL 91 IS 5 AR 055011 DI 10.1103/PhysRevD.91.055011 PG 22 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CD3GD UT WOS:000350965400008 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schofbeck, R Strauss, J Taurok, A Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, M Bansal, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Luyckx, S Ochesanu, S Roland, B Rougny, R De Klundert, MV Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Daci, N Heracleous, N Keaveney, J Lowette, S Maes, M Olbrechts, A Python, Q Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I 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Mohapatra, A. Ojalvo, I. Perry, T. Pierro, G. A. Polese, G. Ross, I. Sarangi, T. Savin, A. Smith, W. H. Vuosalo, C. Woods, N. CA CMS Collaboration TI Measurements of jet multiplicity and differential production cross sections of Z plus jets events in proton-proton collisions at root s=7 TeV SO PHYSICAL REVIEW D LA English DT Article ID PARTON DISTRIBUTIONS; PP COLLISIONS; LHC AB Measurements of differential cross sections are presented for the production of a Z boson and at least one hadronic jet in proton-proton collisions at root s = 7 TeV, recorded by the CMS detector, using a data sample corresponding to an integrated luminosity of 4.9 fb(-1). The jet multiplicity distribution is measured for up to six jets. The differential cross sections are measured as a function of jet transverse momentum and pseudorapidity for the four highest transverse momentum jets. The distribution of the scalar sum of jet transverse momenta is also measured as a function of the jet multiplicity. 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T.; Passaseo, M.; Pazzini, J.; Pegoraro, M.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Vanini, S.; Zotto, P.; Zucchetta, A.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Branca, A.; Dall'Osso, M.; Galanti, M.; Gasparini, F.; Giubilato, P.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Vanini, S.; Zotto, P.; Zucchetta, A.] Univ Padua, Padua, Italy. [Kanishchev, K.] Univ Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Salvini, P.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Menichelli, M.; Romeo, F.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Biasini, M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Menichelli, M.; Romeo, F.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Fiori, F.; Foa, L.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Moon, C. S.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; Fiori, F.; Foa, L.; Ligabue, F.; Vernieri, C.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; D'imperio, G.; Del Re, D.; Diemoz, M.; Grassi, M.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Soffi, L.; Traczyk, P.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; D'imperio, G.; Del Re, D.; Grassi, M.; Longo, E.; Margaroli, F.; Micheli, F.; Nourbakhsh, S.; Rahatlou, S.; Santanastasio, F.; Soffi, L.; Traczyk, P.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Degano, A.; Demaria, N.; Finco, L.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Ortona, G.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Casasso, S.; Costa, M.; Degano, A.; Finco, L.; Migliore, E.; Monaco, V.; Ortona, G.; Pacher, L.; Angioni, G. L. Pinna; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Montanino, D.; Scaini, D.; Schizzi, A.; Umer, T.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Montanino, D.; Scaini, D.; Schizzi, A.; Umer, T.] Univ Trieste, Trieste, Italy. [Kropivnitskaya, A.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Park, H.; Sakharov, A.; Son, D. C.] Kyungpook Natl Univ, Daegu, South Korea. [Kim, T. J.] Chonbuk Natl Univ, Jeonju 561756, South Korea. [Kim, J. Y.; Song, S.] Chonnam Natl Univ, Inst Univ & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, Y.; Lee, B.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, I. C.; Park, S.; Ryu, G.; Ryu, M. S.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, D.; Kwon, E.; Lee, J.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.] Vilnius Univ, Vilnius, Lithuania. [Komaragiri, J. R.; Ali, M. A. B. Md] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; La Cruz, I. Heredia-de; Lopez-Fernandez, R.; Sanchez-Hernandez, A.] Ctr Invest & Estudios Avanzados, IPN, Mexico City, DF, Mexico. [Moreno, S. Carrillo; Valencia, F. Vazquez] Univ Iberoamer, Mexico City, DF, Mexico. [Pedraza, I.; Ibarguen, H. A. Salazar] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Linares, E. Casimiro; Pineda, A. Morelos] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Reucroft, S.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, A.; Ahmad, M.; Hassan, Q.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.; Wolszczak, W.] Univ Warsaw, Fac Phys, Inst Expt Phys, Warsaw, Poland. [Bargassa, P.; Silva, C. Beirao Da Cruz E.; Faccioli, P.; Parracho, P. G. Ferreira; Gallinaro, M.; Nguyen, F.; Antunes, J. Rodrigues; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Golutvin, I.; Karjavin, V.; Konoplyanikov, V.; Korenkov, V.; Kozlov, G.; Lanev, A.; Malakhov, A.; Matveev, V.; Mitsyn, V. V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Shulha, S.; Skatchkov, N.; Smirnov, V.; Tikhonenko, E.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia. [Adzic, P.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Maestre, J. Alcaraz; Battilana, C.; Calvo, E.; Cerrada, M.; Llatas, M. Chamizo; Colino, N.; De La Cruz, B.; Peris, A. Delgado; Vazquez, D. Dominguez; Del Valle, A. Escalante; Bedoya, C. Fernandez; Ramos, J. P. Fernandez; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Lopez, O. Gonzalez; Lopez, S. Goy; Hernandez, J. M.; Josa, M. I.; Merino, G.; De Martino, E. Navarro; Yzquierdo, A. Perez-Calero; Pelayo, J. Puerta; Olmeda, A. Quintario; Redondo, I.; Romero, L.; Soares, M. S.] CIEMAT, E-28040 Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Menendez, J. Fernandez; Folgueras, S.; Caballero, I. Gonzalez; Iglesias, L. Lloret] Univ Oviedo, Oviedo, Spain. [Cifuentes, J. A. Brochero; Cabrillo, I. J.; Calderon, A.; Campderros, J. Duarte; Fernandez, M.; Gomez, G.; Graziano, A.; Virto, A. Lopez; Marco, J.; Marco, R.; Rivero, C. Martinez; Matorras, F.; Sanchez, F. J. Munoz; Gomez, J. Piedra; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Cortabitarte, R. Vilar] Univ Cantabria, CSIC, IFCA, E-39005 Santander, Spain. [Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; David, A.; De Guio, F.; De Roeck, A.; De Visscher, S.; Dobson, M.; Dordevic, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Franzoni, G.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Hansen, M.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Magini, N.; Malgeri, L.; Mannelli, M.; Marrouche, J.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Musella, P.; Orsini, L.; Pape, L.; Perez, E.; Perrozzi, L.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Piparo, D.; Plagge, M.; Racz, A.; Rolandi, G.; Rovere, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Sharma, A.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Steggemann, J.; Stieger, B.; Stoye, M.; Treille, D.; Tsirou, A.; Veres, G. I.; Vlimant, J. R.; Wardle, N.; Woehri, H. K.; Wollny, H.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Bortignon, P.; Buchmann, M. A.; Casal, B.; Chanon, N.; Deisher, A.; Dissertori, G.; Dittmar, M.; Donega, M.; Dunser, M.; Eller, P.; Grab, C.; Hits, D.; Lustermann, W.; Mangano, B.; Marini, A. C.; del Arbol, P. Martinez Ruiz; Meister, D.; Mohr, N.; Nageli, C.; Nessi-Tedaldi, F.; Pandolfi, F.; Pauss, F.; Peruzzi, M.; Quittnat, M.; Rebane, L.; Rossini, M.; Starodumov, A.; Takahashi, M.; Theofilatos, K.; Wallny, R.; Weber, H. A.] ETH, Inst Particle Phys, Zurich, Switzerland. [Amsler, C.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Mejias, B. Millan; Ngadiuba, J.; Robmann, P.; Ronga, F. J.; Taroni, S.; Verzetti, M.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Grundler, U.; Hou, W. -S.; Kao, K. Y.; Lei, Y. J.; Liu, Y. F.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Tzeng, Y. M.; Wilken, R.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Fac Sci, Dept Phys, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Gamsizkan, H.; Karapinar, G.; Ocalan, K.; Sekmen, S.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.] Bogazici Univ, Istanbul, Turkey. [Bahtiyar, H.; Barlas, E.; Cankocak, K.; Vardarli, F. I.; Yucel, M.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Kharkov Phys & Technol Inst, Natl Sci Ctr, UA-310108 Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Womersley, W. J.; Worm, S. D.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Dunne, P.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Hall, G.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Mathias, B.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Lawson, P.; Richardson, C.; Rohlf, J.; Sperka, D.; John, J. St.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Berry, E.; Bhattacharya, S.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.; Swanson, J.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Lander, R.; Miceli, T.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Searle, M.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Cousins, R.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Rakness, G.; Takasugi, E.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Babb, J.; Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Rikova, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Liu, H.; Long, O. R.; Luthra, A.; Malberti, M.; Nguyen, H.; Negrete, M. Olmedo; Shrinivas, A.; Sumowidagdo, S.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Evans, D.; Holzner, A.; Kelley, R.; Klein, D.; Lebourgeois, M.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Palmer, C.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Welke, C.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bradmiller-Feld, J.; Campagnari, C.; Danielson, T.; Dishaw, A.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Incandela, J.; Justus, C.; Mccoll, N.; Richman, J.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Di Marco, E.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Wilkinson, R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Iiyama, Y.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Skinnari, L.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Kaadze, K.; Klima, B.; Kreis, B.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Sharma, S.; Soha, A.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitbeck, A.; Whitmore, J.; Yang, F.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Carver, M.; Cheng, T.; Curry, D.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Field, R. D.; Fisher, M.; Furic, I. K.; Hugon, J.; Konigsberg, J.; Korytov, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Rinkevicius, A.; Shchutska, L.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Haytmyradov, M.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Rahmat, R.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Swartz, M.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Bruner, C.; Gray, J.; Kenny, R. P., III; Malek, M.; Murray, M.; Noonan, D.; Sanders, S.; Sekaric, J.; Stringer, R.; Wang, Q.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Shrestha, S.; Skhirtladze, N.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Belloni, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Bauer, G.; Busza, W.; Cali, I. A.; Chan, M.; Di Matteo, L.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Klute, M.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Ma, T.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Velicanu, D.; Veverka, J.; Wyslouch, B.; Yang, M.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; Gude, A.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Suarez, R. Gonzalez; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Malik, S.; Meier, F.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Dolen, J.; Godshalk, A.; Iashvili, I.; Kharchilava, A.; Kumar, A.; Rappoccio, S.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; Trocino, D.; Wang, R. J.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Hahn, K. A.; Kubik, A.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Brinkerhoff, A.; Chan, K. M.; Drozdetskiy, A.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Pearson, T.; Planer, M.; Ruchti, R.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Puigh, D.; Rodenburg, M.; Smith, G.; Winer, B. L.; Wolfe, H.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Driga, O.; Elmer, P.; Hebda, P.; Hunt, A.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zenz, S. C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Brownson, E.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA. [Alagoz, E.; Barnes, V. E.; Benedetti, D.; Bolla, G.; Bortoletto, D.; De Mattia, M.; Hu, Z.; Jha, M. K.; Jones, M.; Jung, K.; Kress, M.; Leonardo, N.; Pegna, D. Lopes; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shi, X.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.; Stupak, J.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Ecklund, K. M.; Geurts, F. J. M.; Li, W.; Michlin, B.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; Covarelli, R.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Khukhunaishvili, A.; Petrillo, G.; Vishnevskiy, D.] Univ Rochester, Rochester, NY 14627 USA. [Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Lath, A.; Panwalkar, S.; Park, M.; Patel, R.; Salur, S.; Schnetzer, S.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Rose, K.; Spanier, S.; York, A.] Univ Tennessee, Knoxville, TN USA. [Bouhali, O.; Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Khotilovich, V.; Krutelyov, V.; Montalvo, R.; Osipenkov, I.; Pakhotin, Y.; Perloff, A.; Roe, J.; Rose, A.; Safonov, A.; Sakuma, T.; Suarez, I.; Tatarinov, A.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kovitanggoon, K.; Kunori, S.; Lee, S. W.; Libeiro, T.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Johns, W.; Maguire, C.; Mao, Y.; Melo, A.; Sharma, M.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN 37235 USA. [Arenton, M. W.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Li, H.; Lin, C.; Neu, C.; Wood, J.] Univ Virginia, Charlottesville, VA USA. [Clarke, C.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sturdy, J.] Wayne State Univ, Detroit, MI USA. [Belknap, D. A.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Dodd, L.; Duric, S.; Friis, E.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Lanaro, A.; Lazaridis, C.; Levine, A.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ross, I.; Sarangi, T.; Savin, A.; Smith, W. H.; Vuosalo, C.; Woods, N.] Univ Wisconsin, Madison, WI 53706 USA. [Fabjan, C.; Fruehwirth, R.; Jeitler, M.; Krammer, M.; Wulz, C. -E.] Vienna Univ Technol, A-1040 Vienna, Austria. [Rabady, D.; Pernie, L.; Genchev, V.; Boudoul, G.; Contardo, D.; Lingemann, J.; Mohanty, A. K.; Radogna, R.; Silvestris, L.; Masetti, G.; Giordano, F.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Lucchini, M. T.; Cavallo, N.; Di Guida, S.; Meola, S.; Paolucci, P.; Spiezia, A.; Palla, F.; Vernieri, C.; Micheli, F.; Soffi, L.; Argiro, S.; Casasso, S.; Obertino, M. M.; Schizzi, A.; Stickland, D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Beluffi, C.] Univ Haute Alsace Mulhouse, Univ Strasbourg, Inst Pluridisciplinaire Hubert Curien, CNRS IN2P3, Strasbourg, France. [Giammanco, A.; Hartmann, F.; Hauth, T.; Kornmayer, A.] NICPB, Tallinn, Estonia. [Popov, A.; Zhukov, V.; Katkov, I.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Chinellato, J.; Manganote, E. J. Tonelli] Univ Estadual Campinas, Campinas, SP, Brazil. [Plestina, R.; Bernet, C.] Ecole Polytech, IN2P3 CNRS, Lab Leprince Ringuet, Palaiseau, France. [Finger, M., Jr.; Tsamalaidze, Z.] Joint Inst Nucl Res, Dubna, Russia. [Assran, Y.] Suez Univ, Suez, Egypt. [Kamel, A. Ellithi] Cairo Univ, Cairo, Egypt. [Mahmoud, M. A.] Fayoum Univ, Al Fayyum, Egypt. [Radi, A.] British Univ Egypt, Cairo, Egypt. [Radi, A.] Ain Shams Univ, Cairo, Egypt. [Agram, J. -L.; Conte, E.; Fontaine, J. -C.] Univ Haute Alsace, Mulhouse, France. [Bergholz, M.; Lohmann, W.; Schmidt, R.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Horvath, D.] Inst Nucl Res, ATOMKI, H-4001 Debrecen, Hungary. [Vesztergombi, G.; Veres, G. I.] Eotvos Lorand Univ, Budapest, Hungary. [Karancsi, J.] Univ Debrecen, Debrecen, Hungary. [Bhowmik, S.; Maity, M.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Gurtu, A.] King Abdulaziz Univ, Jeddah 21413, Saudi Arabia. [Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka. [Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Fahim, A.] Sharif Univ Technol, Tehran, Iran. [Safarzadeh, B.] Islamic Azad Univ, Plasma Phys Res Ctr, Sci & Res Branch, Tehran, Iran. [Biasotto, M.] Ist Nazl Fis Nucl, Lab Nazl Legnaro, I-35020 Legnaro, Italy. [Androsov, K.; Ciocci, M. A.; Grippo, M. T.] Univ Siena, I-53100 Siena, Italy. [Moon, C. S.] CNRS, IN2P3, Paris, France. Purdue Univ, W Lafayette, IN 47907 USA. [La Cruz, I. Heredia-de] Univ Michoacana, Morelia, Michoacan, Mexico. [Matveev, V.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Kim, V.] St Petersburg State Polytech Univ, St Petersburg, Russia. [Dubinin, M.] CALTECH, Pasadena, CA 91125 USA. [Adzic, P.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Colafranceschi, S.] Univ Rome, Fac Ingn, Rome, Italy. [Rolandi, G.] Ist Nazl Fis Nucl, Scuola Normale & Sez, Pisa, Italy. [Sphicas, P.] Univ Athens, Athens, Greece. [Nageli, C.] Paul Scherrer Inst, Villigen, Switzerland. [Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Bakirci, M. N.; Ozturk, S.; Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey. [Cerci, S.; Cerci, D. Sunar; Tali, B.] Adiyaman Univ, Adiyaman, Turkey. [Ozdemir, K.] Cag Univ, Mersin, Turkey. [Sogut, K.] Mersin Univ, Mersin, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Kaya, M.] Marmara Univ, Istanbul, Turkey. [Kaya, O.] Kafkas Univ, Kars, Turkey. [Bahtiyar, H.; Albayrak, E. A.; Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Newbold, D. M.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Bilki, B.] Argonne Natl Lab, Argonne, IL 60439 USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Yetkin, T.; Kamon, T.] Yildiz Tekn Univ, Istanbul, Turkey. [Bouhali, O.] Texas A&M Univ, Doha, Qatar. Kyungpook Natl Univ, Daegu, South Korea. RP Khachatryan, V (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Goh, Junghwan/Q-3720-2016; Ruiz, Alberto/E-4473-2011; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Paulini, Manfred/N-7794-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Ogul, Hasan/S-7951-2016; Hernandez Calama, Jose Maria/H-9127-2015; ciocci, maria agnese /I-2153-2015; Bedoya, Cristina/K-8066-2014; My, Salvatore/I-5160-2015; Benussi, Luigi/O-9684-2014; Lo Vetere, Maurizio/J-5049-2012; Ragazzi, Stefano/D-2463-2009; Grandi, Claudio/B-5654-2015; Rovelli, Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; Dogra, Sunil /B-5330-2013; Hoorani, Hafeez/D-1791-2013; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Da Silveira, Gustavo Gil/N-7279-2014; Mora Herrera, Maria Clemencia/L-3893-2016; Mundim, Luiz/A-1291-2012; Haj Ahmad, Wael/E-6738-2016; Konecki, Marcin/G-4164-2015; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Calderon, Alicia/K-3658-2014; Cerrada, Marcos/J-6934-2014; Perez-Calero Yzquierdo, Antonio/F-2235-2013; Novaes, Sergio/D-3532-2012; Della Ricca, Giuseppe/B-6826-2013; Chinellato, Jose Augusto/I-7972-2012; Tomei, Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Tinoco Mendes, Andre David/D-4314-2011; Seixas, Joao/F-5441-2013; Leonidov, Andrey/M-4440-2013; Andreev, Vladimir/M-8665-2015; Cakir, Altan/P-1024-2015; Matorras, Francisco/I-4983-2015; Gennai, Simone/P-2880-2015; TUVE', Cristina/P-3933-2015; Dudko, Lev/D-7127-2012; Paganoni, Marco/A-4235-2016; Azarkin, Maxim/N-2578-2015; de Jesus Damiao, Dilson/G-6218-2012; Horani, Hafeez /L-2414-2015; Calvo Alamillo, Enrique/L-1203-2014; Flix, Josep/G-5414-2012; Cavallo, Nicola/F-8913-2012; Montanari, Alessandro/J-2420-2012; Manganote, Edmilson/K-8251-2013; Lokhtin, Igor/D-7004-2012; Bernardes, Cesar Augusto/D-2408-2015; VARDARLI, Fuat Ilkehan/B-6360-2013; Sen, Sercan/C-6473-2014; D'Alessandro, Raffaello/F-5897-2015; Petrushanko, Sergey/D-6880-2012; Wulz, Claudia-Elisabeth/H-5657-2011; Belyaev, Alexander/F-6637-2015; Stahl, Achim/E-8846-2011; Trocsanyi, Zoltan/A-5598-2009 OI Goh, Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787; Ogul, Hasan/0000-0002-5121-2893; Hernandez Calama, Jose Maria/0000-0001-6436-7547; ciocci, maria agnese /0000-0003-0002-5462; Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680; Benussi, Luigi/0000-0002-2363-8889; Lo Vetere, Maurizio/0000-0002-6520-4480; Ragazzi, Stefano/0000-0001-8219-2074; Grandi, Claudio/0000-0001-5998-3070; Rovelli, Tiziano/0000-0002-9746-4842; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Mundim, Luiz/0000-0001-9964-7805; Haj Ahmad, Wael/0000-0003-1491-0446; Konecki, Marcin/0000-0001-9482-4841; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Cerrada, Marcos/0000-0003-0112-1691; Perez-Calero Yzquierdo, Antonio/0000-0003-3036-7965; Novaes, Sergio/0000-0003-0471-8549; Della Ricca, Giuseppe/0000-0003-2831-6982; Chinellato, Jose Augusto/0000-0002-3240-6270; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Seixas, Joao/0000-0002-7531-0842; Matorras, Francisco/0000-0003-4295-5668; TUVE', Cristina/0000-0003-0739-3153; Dudko, Lev/0000-0002-4462-3192; Paganoni, Marco/0000-0003-2461-275X; de Jesus Damiao, Dilson/0000-0002-3769-1680; Calvo Alamillo, Enrique/0000-0002-1100-2963; Flix, Josep/0000-0003-2688-8047; Montanari, Alessandro/0000-0003-2748-6373; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Belyaev, Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279 FU Austrian Federal Ministry of Science, Research and Economy; Austrian Science Fund; Belgian Fonds de la Recherche Scientifique; Fonds voor Wetenschappelijk Onderzoek; Brazilian Funding Agency (CNPq); Brazilian Funding Agency (CAPES); Brazilian Funding Agency (FAPERJ); Brazilian Funding Agency (FAPESP); Bulgarian Ministry of Education and Science; CERN; Chinese Academy of Sciences; Ministry of Science and Technology; National Natural ScienceFoundationofChina; Colombian FundingAgency (COLCIENCIAS); Croatian Ministry of Science, Education, and Sport; Croatian Science Foundation; Research Promotion Foundation, Cyprus; Ministry of Education and Research, Estonia; Estonian Research Council, Estonia [IUT23-4, IUT23-6]; European Regional Development Fund, Estonia; Academy of Finland; Finnish Ministry of Education and Culture; Helsinki Institute of Physics; Institut National de Physique Nucleaire et de Physique des Particules / CNRS, France; Commissariat a l'Energie Atomique et aux Energies Alternatives / CEA, France; Bundesministerium fur Bildung und Forschung, Germany; Deutsche Forschungsgemeinschaft, Germany; Helmholtz-Gemeinschaft Deutscher Forschungs zentren, Germany; General Secretariat for Research and Technology, Greece; National Scientific Research Foundation, Hungary; National Innovation Office, Hungary; Department of Atomic Energy, India; Department of Science and Technology, India; Institute for Studies in Theoretical Physics and Mathematics, Iran; Science Foundation, Ireland; Istituto Nazionale di Fisica Nucleare, Italy; Korean Ministry of Education, Science and Technology, Republic of Korea; World Class University program of NRF, Republic of Korea; Lithuanian Academy of Sciences; Ministry of Education, and University of Malaya (Malaysia); Mexican Funding Agency (CINVESTAV); Mexican Funding Agency (CONACYT); Mexican Funding Agency (SEP); Mexican Funding Agency (UASLP-FAI); Ministry of Business, Innovation and Employment, New Zealand; Pakistan Atomic Energy Commission; Ministry of Science and Higher Education, Poland; National Science Centre, Poland; Fundacao para a Cienciaea Tecnologia, Portugal; JINR, Dubna; Ministry of Education and Science of the Russian Federation; Federal Agency of Atomic Energy of the Russian Federation; Russian Academy of Sciences; Russian Foundation for Basic Research; Ministry of Education, Science and Technological Development of Serbia; Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio, Spain; Swiss Funding Agency (ETH Board); Swiss Funding Agency (ETH Zurich); Swiss Funding Agency (PSI); Swiss Funding Agency (SNF); Swiss Funding Agency (UniZH); Swiss Funding Agency (Canton Zurich); Swiss Funding Agency (SER); Ministry of Science and Technology, Taipei; Thailand Center of Excellence in Physics; Institute for the Promotion of Teaching Science andTechnologyofThailand; SpecialTaskForceforActivating Research; National Science and Technology Development Agency of Thailand; Scientific and Technical Research Council of Turkey; Turkish Atomic Energy Authority; National Academy of Sciences of Ukraine, Ukraine; State Fund for Fundamental Researches, Ukraine; Science and Technology Facilities Council, United Kingdom; U.S. Department of Energy; U.S. National Science Foundation; Marie Curie program; European Research Council; EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council ofScienceandIndustrialResearch, India; HOMINGPLUS program of Foundation for Polish Science; European Union; Regional Development Fund; Compagnia di San Paolo (Torino); Consorzio per la Fisica (Trieste); MIUR (Italy) [20108T4XTM]; Thalis and Aristeia programs; EU-ESF; GreekNSRF; NationalPrioritiesResearchProgram by Qatar National Research Fund FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of theCMS effort. In addition, wegratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: the Austrian Federal Ministry of Science, Research and Economy and the Austrian Science Fund; the Belgian Fonds de la Recherche Scientifique, and Fonds voor Wetenschappelijk Onderzoek; the Brazilian Funding Agencies (CNPq, CAPES, FAPERJ, and FAPESP); the Bulgarian Ministry of Education and Science; CERN; the Chinese Academy of Sciences, Ministry of Science and Technology, and National Natural ScienceFoundationofChina; theColombian FundingAgency (COLCIENCIAS); the Croatian Ministry of Science, Education, and Sport, and the Croatian Science Foundation; the Research Promotion Foundation, Cyprus; the Ministry of Education and Research, Estonian Research Council via Grants No. IUT23-4 and No.; IUT23-6 and European Regional Development Fund, Estonia; the Academy of Finland, Finnish Ministry of Education and Culture, and Helsinki Institute of Physics; the Institut National de Physique Nucleaire et de Physique des Particules / CNRS, and Commissariat a l'Energie Atomique et aux Energies Alternatives / CEA, France; the Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft, and Helmholtz-Gemeinschaft Deutscher Forschungs zentren, Germany; the General Secretariat for Research and Technology, Greece; the National Scientific Research Foundation, and National Innovation Office, Hungary; the Department of Atomic Energy and the Department of Science and Technology, India; the Institute for Studies in Theoretical Physics and Mathematics, Iran; the Science Foundation, Ireland; the Istituto Nazionale di Fisica Nucleare, Italy; the Korean Ministry of Education, Science and Technology and the World Class University program of NRF, Republic of Korea; the Lithuanian Academy of Sciences; the Ministry of Education, and University of Malaya (Malaysia); the Mexican Funding Agencies (CINVESTAV, CONACYT, SEP, and UASLP-FAI); the Ministry of Business, Innovation and Employment, New Zealand; the Pakistan Atomic Energy Commission; the Ministry of Science and Higher Education and the National Science Centre, Poland; the Fundacao para a Cienciaea Tecnologia, Portugal; JINR, Dubna; the Ministry of Education and Science of the Russian Federation, the Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences, and the Russian Foundation for Basic Research; the Ministry of Education, Science and Technological Development of Serbia; the Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio 2010, Spain; the Swiss Funding Agencies (ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER); the Ministry of Science and Technology, Taipei; the Thailand Center of Excellence in Physics, the Institute for the Promotion of Teaching Science andTechnologyofThailand, SpecialTaskForceforActivating Research and the National Science and Technology Development Agency of Thailand; the Scientific and Technical Research Council of Turkey, and Turkish Atomic Energy Authority; the National Academy of Sciences of Ukraine, and State Fund for Fundamental Researches, Ukraine; the Science and Technology Facilities Council, United Kingdom; the U.S. Department of Energy, and the U.S. National Science Foundation. Individuals have received support from the Marie Curie program and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council ofScienceandIndustrialResearch, India; theHOMINGPLUS program of Foundation for Polish Science, cofinanced by the European Union, Regional Development Fund; the Compagnia di San Paolo (Torino); the Consorzio per la Fisica (Trieste); MIUR Grant No. 20108T4XTM (Italy); the Thalis and Aristeia programs cofinanced by EU-ESF and theGreekNSRF; andtheNationalPrioritiesResearchProgram by Qatar National Research Fund. NR 57 TC 6 Z9 6 U1 9 U2 58 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD MAR 11 PY 2015 VL 91 IS 5 AR 052008 DI 10.1103/PhysRevD.91.052008 PG 26 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CD3GD UT WOS:000350965400001 ER PT J AU Hau-Riege, S Weisheit, J AF Hau-Riege, Stefan Weisheit, Jon TI Electric microfields in dense carbon-hydrogen plasmas SO PHYSICAL REVIEW E LA English DT Article ID COUPLED 2-COMPONENT PLASMAS; FIELD DISTRIBUTIONS; MOLECULAR-DYNAMICS; LINE-SHAPES; IONIZED GAS; SIMULATIONS; SYSTEMS; LASER; FLUCTUATIONS; COMPONENT AB Classical molecular dynamics is used to investigate stationary and time-dependent properties of microfields in hot, solid density, electron-ion plasmas. Even at the high temperatures considered here, such simulations require quantum statistical potentials (QSPs) to mimic the essential effects of diffraction and exchange symmetry for electrons. Fortunately, key results relevant to microfield distributions are found to be insensitive to different, plausible QSP choices. Atomic processes in plasmas will depend on the time average of the microfields. It is not clear, a priori, what the time duration of this average should be. The question of how best to extract the quasistatic (low-frequency) microfield from a classical molecular dynamics simulation is explored in some detail, and the time-averaging approach we adopt involves both plasma and atomic time scale constraints. One of the major findings described in the paper is that for a large time interval, the time-averaged microfield does not significantly change. Our discussion of this suite of large simulations for plasma mixtures focuses on understanding various features and trends revealed by data for C-H plasmas having carbon fractions ranging from 0.01 to 1, and different temperatures well above T-Fermi. C1 [Hau-Riege, Stefan] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Weisheit, Jon] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. RP Hau-Riege, S (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX We thank Dr. C. A. Iglesias for useful discussions, and our Cimarron colleagues for their continued interest and suggestions. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 57 TC 1 Z9 1 U1 4 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD MAR 11 PY 2015 VL 91 IS 3 AR 033106 DI 10.1103/PhysRevE.91.033106 PG 11 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA CD3GO UT WOS:000350966600015 PM 25871223 ER PT J AU Neish, MJ Oxley, MP Guo, J Sales, BC Allen, LJ Chisholm, MF AF Neish, M. J. Oxley, M. P. Guo, J. Sales, B. C. Allen, L. J. Chisholm, M. F. TI Local Observation of the Site Occupancy of Mn in a MnFePSi Compound SO PHYSICAL REVIEW LETTERS LA English DT Article ID MAGNETOCALORIC MATERIALS; MAGNETIC-STRUCTURE; SINGLE-CRYSTALS; STEM; EELS; OXIDES AB MnFePSi compounds are promising materials for magnetic refrigeration as they exhibit a giant magnetocaloric effect. From first principles calculations and experiments on bulk materials, it has been proposed that this is due to the Mn and Fe atoms preferentially occupying two different sites within the atomic lattice. A recently developed technique was used to deconvolve the obscuring effects of both multiple elastic scattering and thermal diffuse scattering of the probe in an atomic resolution electron energy-loss spectroscopy investigation of a MnFePSi compound. This reveals, unambiguously, that the Mn atoms preferentially occupy the 3g site in a hexagonal crystal structure, confirming the theoretical predictions. After deconvolution, the data exhibit a difference in the Fe L-2,L-3 ratio between the 3f and 3g sites consistent with differences in magnetic moments calculated from first principles, which are also not observed in the raw data. C1 [Neish, M. J.; Allen, L. J.] Univ Melbourne, Sch Phys, Parkville, Vic 3010, Australia. [Oxley, M. P.; Sales, B. C.; Chisholm, M. F.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Oxley, M. P.] Vanderbilt Univ, Dept Phys & Astron, Nashville, TN 37212 USA. [Guo, J.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. RP Neish, MJ (reprint author), Univ Melbourne, Sch Phys, Parkville, Vic 3010, Australia. EM lja@unimelb.edu.au RI guo, junjie/I-3189-2012 OI guo, junjie/0000-0002-3414-3734 FU Australian Research Council [DP110102228]; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; DOE [DE-FG02-09R46554] FX This research was supported under the Discovery Projects funding scheme of the Australian Research Council (Project No. DP110102228). This work was sponsored by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division and supported in part by DOE Grant No. DE-FG02-09R46554. NR 33 TC 5 Z9 5 U1 9 U2 76 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 11 PY 2015 VL 114 IS 10 AR 106101 DI 10.1103/PhysRevLett.114.106101 PG 5 WC Physics, Multidisciplinary SC Physics GA CD3GQ UT WOS:000350966800013 PM 25815950 ER PT J AU Sandoval, L Perez, D Uberuaga, BP Voter, AF AF Sandoval, Luis Perez, Danny Uberuaga, Blas P. Voter, Arthur F. TI Competing Kinetics and He Bubble Morphology in W SO PHYSICAL REVIEW LETTERS LA English DT Article ID LOW-ENERGY HELIUM; MOLECULAR-DYNAMICS SIMULATION; DISLOCATION LOOP; FREE SURFACE; TUNGSTEN SURFACES; HYDROGEN; METALS; IRRADIATION; CASCADES; CLUSTERS AB The growth process of He bubbles in W is investigated using molecular dynamics and parallel replica dynamics for growth rates spanning 6 orders of magnitude. Fast and slow growth regimes are defined relative to typical diffusion hopping times of W interstitials around the He bubble. Slow growth rates allow the diffusion of interstitials around the bubble, favoring the biased growth of the bubble towards the surface. In contrast, at fast growth rates interstitials do not have time to diffuse around the bubble, leading to a more isotropic growth and increasing the surface damage. C1 [Sandoval, Luis; Perez, Danny; Voter, Arthur F.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Uberuaga, Blas P.] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. RP Sandoval, L (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RI Sandoval, Luis/B-2221-2009; OI Sandoval, Luis/0000-0002-1172-7972; Voter, Arthur/0000-0001-9788-7194 FU U.S. DOE, Office of Science, Office of Fusion Energy Sciences, and Office of Advanced Scientific Computing Research through the Scientific Discovery through Advanced Computing (SciDAC); U.S. DOE, Office of Basic Energy Sciences, Materials Sciences and Engineering Division; Office of Science of the U.S. DOE [DE-AC02-05CH11231, DE-AC05-00OR22725]; Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. DOE [DE-AC52-O6NA25396] FX The authors would like to thank Brian Wirth and Chun-Yaung (Albert) Lu for the useful discussion. L. S., D. P., and B. P. U. acknowledge support by the U.S. DOE, Office of Science, Office of Fusion Energy Sciences, and Office of Advanced Scientific Computing Research through the Scientific Discovery through Advanced Computing (SciDAC) project on Plasma-Surface Interactions. A. F. V. was supported by the U.S. DOE, Office of Basic Energy Sciences, Materials Sciences and Engineering Division. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. DOE under Contract No. DE-AC02-05CH11231, and resources of the Oak Ridge Leadership Computing Facility at Oak Ridge National Laboratory, which is supported by the Office of Science of the U.S. DOE under Contract No. DE-AC05-00OR22725. Los Alamos National Laboratory is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. DOE, under Contract No. DE-AC52-O6NA25396. NR 37 TC 19 Z9 19 U1 5 U2 44 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 11 PY 2015 VL 114 IS 10 AR 105502 DI 10.1103/PhysRevLett.114.105502 PG 5 WC Physics, Multidisciplinary SC Physics GA CD3GQ UT WOS:000350966800010 PM 25815946 ER PT J AU Wang, YT Liu, Y Wang, G Anwand, W Jenkins, CA Arenholz, E Munnik, F Gordan, OD Salvan, G Zahn, DRT Chen, XL Gemming, S Helm, M Zhou, SQ AF Wang, Yutian Liu, Yu Wang, Gang Anwand, Wolfgang Jenkins, Catherine A. Arenholz, Elke Munnik, Frans Gordan, Ovidiu D. Salvan, Georgeta Zahn, Dietrich R. T. Chen, Xiaolong Gemming, Sibylle Helm, Manfred Zhou, Shengqiang TI Carbon p Electron Ferromagnetism in Silicon Carbide SO SCIENTIFIC REPORTS LA English DT Article ID POINT-DEFECTS; SPIN QUBITS; PRINCIPLES; ABSORPTION; MAGNETISM; GRAPHENE AB Ferromagnetism can occur in wide-band gap semiconductors as well as in carbon-based materials when specific defects are introduced. It is thus desirable to establish a direct relation between the defects and the resulting ferromagnetism. Here, we contribute to revealing the origin of defect-induced ferromagnetism using SiC as a prototypical example. We show that the long-range ferromagnetic coupling can be attributed to the p electrons of the nearest-neighbor carbon atoms around the VSiVC divacancies. Thus, the ferromagnetism is traced down to its microscopic electronic origin. C1 [Wang, Yutian; Liu, Yu; Munnik, Frans; Gemming, Sibylle; Helm, Manfred; Zhou, Shengqiang] Helmholtz Zentrum Dresden Rossendorf, Inst Ion Beam Phys & Mat Res, D-01328 Dresden, Germany. [Liu, Yu; Wang, Gang; Chen, Xiaolong] Chinese Acad Sci, Inst Phys, Beijing Natl Lab Condensed Matter Phys, Res & Dev Ctr Funct Crystals, Beijing 100190, Peoples R China. [Anwand, Wolfgang] Helmholtz Zentrum Dresden Rossendorf, Inst Radiat Phys, D-01328 Dresden, Germany. [Jenkins, Catherine A.; Arenholz, Elke] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Helm, Manfred] Tech Univ Dresden, D-01062 Dresden, Germany. [Gordan, Ovidiu D.; Salvan, Georgeta; Zahn, Dietrich R. T.; Gemming, Sibylle] Tech Univ Chemnitz, Inst Phys, D-09107 Chemnitz, Germany. RP Liu, Y (reprint author), Helmholtz Zentrum Dresden Rossendorf, Inst Ion Beam Phys & Mat Res, Bautzner Landstr 400, D-01328 Dresden, Germany. EM y.liu@hzdr.de; s.zhou@hzdr.de RI Liu, Yu/A-1018-2012; Zhou, Shengqiang/C-1497-2009; Helm, Manfred/B-2284-2009; Salvan, Georgeta/O-8084-2015; Wang, Gang/F-1858-2011; OI Zhou, Shengqiang/0000-0002-4885-799X; Salvan, Georgeta/0000-0002-2565-9675; Zahn, Dietrich RT/0000-0002-8455-4582 FU Helmholtz-Gemeinschaft Deutscher Forschungszentren [VH-NG-713, VH-VI-442, VH-PD-146]; China Scholarship Council [2010675001]; U.S. Department of Energy [DE-AC02-05CH11231]; National Natural Science Foundation of China [51322211, 90922037, 51072222, 51272276] FX The work is financially supported by the Helmholtz-Gemeinschaft Deutscher Forschungszentren (VH-NG-713, VH-VI-442 and VH-PD-146). Y. Wang thanks the China Scholarship Council (File No. 2010675001) for supporting his stay at HZDR. The Advanced Light Source is supported by the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. G. Wang, and X. L. Chen also thank the support by the National Natural Science Foundation of China (Grant Nos. 51322211, 90922037, 51072222 and 51272276). NR 39 TC 9 Z9 9 U1 2 U2 52 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAR 11 PY 2015 VL 5 AR 8999 DI 10.1038/srep08999 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CD5OS UT WOS:000351138300014 PM 25758040 ER PT J AU Matt, G Balokovic, M Marinucci, A Ballantyne, DR Boggs, SE Christensen, FE Comastri, A Craig, WW Gandhi, P Hailey, CJ Harrison, FA Madejski, G Madsen, KK Stern, D Zhang, WW AF Matt, G. Balokovic, M. Marinucci, A. Ballantyne, D. R. Boggs, S. E. Christensen, F. E. Comastri, A. Craig, W. W. Gandhi, P. Hailey, C. J. Harrison, F. A. Madejski, G. Madsen, K. K. Stern, D. Zhang, W. W. TI The hard X-ray spectrum of NGC 5506 as seen by NuSTAR SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE accretion, accretion discs; galaxies: active; galaxies: individual: NGC 5506 ID ACTIVE GALACTIC NUCLEI; XMM-NEWTON; IC 4329A; LINE; REFLECTION; NGC-5506; SPECTROSCOPY; GALAXIES AB NuSTAR observed the bright Compton-thin, narrow-line Seyfert 1 galaxy, NGC 5506, for about 56 ks. In agreement with past observations, the spectrum is well fitted by a power law with Gamma similar to 1.9, a distant reflection component and narrow ionized iron lines. A relativistically blurred reflection component is not required by the data. When an exponential high-energy cutoff is added to the power law, a value of 720(-190)(+130) keV (90 per cent confidence level) is found. Even allowing for systematic uncertainties, we find a 3 sigma lower limit to the high-energy cutoff of 350 keV, the highest lower limit to the cutoff energy found so far in an AGN by NuSTAR. C1 [Matt, G.; Marinucci, A.] Univ Rome Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Balokovic, M.; Harrison, F. A.; Madsen, K. K.] CALTECH, Cahill Ctr Astron & Astrophys, Pasadena, CA 91125 USA. [Ballantyne, D. R.] Georgia Inst Technol, Sch Phys, Ctr Relativist Astrophys, Atlanta, GA 30332 USA. [Boggs, S. E.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Christensen, F. E.; Craig, W. W.] Tech Univ Denmark, DTU Space Natl Space Inst, DK-2800 Lyngby, Denmark. [Comastri, A.] INAF Osservatorio Astron Bologna, I-40127 Bologna, Italy. [Craig, W. W.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Gandhi, P.] Univ Durham, Dept Phys, Durham DH1 3LE, England. [Gandhi, P.] Univ Southampton, Sch Phys & Astron, Southampton SO17 1BJ, Hants, England. [Hailey, C. J.] Columbia Univ, Columbia Astrophys Lab, New York, NY 10027 USA. [Madejski, G.] SLAC Natl Accelerator Lab, Kavli Inst Particle Astrophys & Cosmol, Menlo Pk, CA 94025 USA. [Stern, D.] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Zhang, W. W.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. RP Matt, G (reprint author), Univ Rome Tre, Dipartimento Matemat & Fis, Via Vasca Navale 84, I-00146 Rome, Italy. EM matt@fis.uniroma3.it RI Boggs, Steven/E-4170-2015 OI Boggs, Steven/0000-0001-9567-4224 FU National Aeronautics and Space Administration; Italian Space Agency [ASI/INAF I/037/12/0-011/13]; European Union [312789]; Fulbright International Science and Technology Award FX This work has made use of data from the NuSTAR mission, a project led by the California Institute of Technology, managed by the Jet Propulsion Laboratory, and funded by the National Aeronautics and Space Administration. We thank the NuSTAR Operations, Software and Calibration teams for support with the execution and analysis of these observations. This research has made use of the NuSTAR Data Analysis Software (NUSTARDAS) jointly developed by the ASI Science Data Center (ASDC, Italy) and the California Institute of Technology (USA). GM, AM and AC acknowledge financial support from Italian Space Agency under grant ASI/INAF I/037/12/0-011/13. GM and AM also acknowledge financial support from the European Union Seventh Framework Programme (FP7/2007-2013) under grant agreement no. 312789. MB acknowledges support from the Fulbright International Science and Technology Award. NR 24 TC 12 Z9 12 U1 0 U2 5 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD MAR 11 PY 2015 VL 447 IS 4 BP 3029 EP 3033 DI 10.1093/mnras/stu2653 PG 5 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CC3TR UT WOS:000350273400004 ER PT J AU Jones, S Hirschi, R Pignatari, M Heger, A Georgy, C Nishimura, N Fryer, C Herwig, F AF Jones, S. Hirschi, R. Pignatari, M. Heger, A. Georgy, C. Nishimura, N. Fryer, C. Herwig, F. TI Code dependencies of pre-supernova evolution and nucleosynthesis in massive stars: evolution to the end of core helium burning SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE stars: abundances; stars: evolution; stars: interiors; stars: massive; supernovae: general; galaxies: abundances ID S-PROCESS NUCLEOSYNTHESIS; M-CIRCLE-DOT; EQUATION-OF-STATE; THERMONUCLEAR REACTION-RATES; NEUTRINO-DRIVEN SUPERNOVAE; STELLAR ASTROPHYSICS MESA; X-RAY-BURSTS; COLLAPSE SUPERNOVAE; PRESUPERNOVA EVOLUTION; COMPTON-SCATTERING AB Massive stars are key sources of radiative, kinetic and chemical feedback in theUniverse. Grids of massive star models computed by different groups each using their own codes, input physics choices and numerical approximations, however, lead to inconsistent results for the same stars. We use three of these 1D codes - GENEC, KEPLER and MESA - to compute non-rotating stellar models of 15, 20 and 25M(circle dot) and compare their nucleosynthesis. We follow the evolution from the main sequence until the end of core helium burning. The GENEC and KEPLER models hold physics assumptions used in large grids of published models. The MESA code was set up to use convective core overshooting such that the CO core masses are consistent with those obtained by GENEC. For all models, full nucleosynthesis is computed using the NuGrid post-processing tool MPPNP. We find that the surface abundances predicted by the models are in reasonable agreement. In the helium core, the standard deviation of the elemental overproduction factors for Fe to Mo is less than 30 per cent - smaller than the impact of the present nuclear physics uncertainties. For our three initial masses, the three stellar evolution codes yield consistent results. Differences in key properties of the models, e.g. helium and CO core masses and the time spent as a red supergiant, are traced back to the treatment of convection and, to a lesser extent, mass loss. The mixing processes in stars remain the key uncertainty in stellar modelling. Better constrained prescriptions are thus necessary to improve the predictive power of stellar evolution models. C1 [Jones, S.; Herwig, F.] Univ Victoria, Dept Phys & Astron, Victoria, BC V8W 3P6, Canada. [Jones, S.; Hirschi, R.; Georgy, C.; Nishimura, N.] Keele Univ, Astrophys Grp, Keele ST5 5BG, Staffs, England. [Hirschi, R.] Univ Tokyo, Kavli Inst Phys & Math Universe WPI, Kashiwa, Chiba 2778583, Japan. [Pignatari, M.] Univ Basel, Dept Phys, CH-4056 Basel, Switzerland. [Heger, A.] Monash Univ, Sch Math Sci, Monash Ctr Astrophys, Clayton, Vic 3800, Australia. [Heger, A.] Univ Minnesota, Sch Phys & Astron, Minnesota Inst Astrophys, Minneapolis, MN 55455 USA. [Heger, A.; Herwig, F.] Univ Notre Dame, Joint Inst Nucl Astrophys, Notre Dame, IN 46556 USA. [Fryer, C.] Los Alamos Natl Lab, Computat Phys & Methods CCS 2, Los Alamos, NM 87545 USA. RP Jones, S (reprint author), NuGrid Collaborat, London, England. EM swjones@uvic.ca RI Georgy, Cyril/B-4476-2016; OI Georgy, Cyril/0000-0003-2362-4089; Nishimura, Nobuya/0000-0002-0842-7856 FU NSF [PHY 02-16783, PHY 09-22648, AST-1109394]; Eurocore project Eurogenesis; ERC Starting Grant [306901]; World Premier International Research Center Initiative (WPI Initiative), MEXT, Japan; Ambizione grant of the SNSF; SNF grant (Switzerland); US DOE [FC02-09ER41618, DE-FG02-87ER40328]; ARC Future Fellowship [FT120100363] FX NuGrid acknowledges significant support from NSF grants PHY 02-16783 and PHY 09-22648 (Joint Institute for Nuclear Astrophysics, JINA). RH and CG acknowledge the support from Eurocore project Eurogenesis and ERC Starting Grant No. 306901. RH acknowledges support from the World Premier International Research Center Initiative (WPI Initiative), MEXT, Japan. MP acknowledges the support from the Ambizione grant of the SNSF and the SNF grant (Switzerland). AH acknowledges the support by NSF through grant AST-1109394, by US DOE grants FC02-09ER41618 (Sci-DAC), DE-FG02-87ER40328 and by an ARC Future Fellowship (FT120100363). NR 106 TC 13 Z9 13 U1 1 U2 3 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD MAR 11 PY 2015 VL 447 IS 4 BP 3115 EP 3129 DI 10.1093/mnras/stu2657 PG 15 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CC3TR UT WOS:000350273400012 ER PT J AU Asner, DM Burns, K Campbell, LW Greenfield, B Kos, MS Orrell, JL Schram, M VanDevender, B Wood, LS Wootan, DW AF Asner, D. M. Burns, K. Campbell, L. W. Greenfield, B. Kos, M. S. Orrell, J. L. Schram, M. VanDevender, B. Wood, L. S. Wootan, D. W. TI Method of fission product beta spectra measurements for predicting reactor anti-neutrino emission SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Proton beam; Beta decay; Anti-neutrinos; Reactor anomaly ID PU-239 AB The nuclear fission process that occurs in the core of nuclear reactors results in unstable, neutron-rich fission products that subsequently beta decay and emit electron antineutrinos. These reactor neutrinos have served neutrino physics research from the initial discovery of the neutrino to today's precision measurements of neutrino mixing angles. The prediction of the absolute flux and energy spectrum of the emitted reactor neutrinos hinges upon a series of seminal papers based on measurements performed in the 1970s and 1980s, The steadily improving reactor neutrino measurement techniques and recent reconsiderations of the agreement between the predicted and observed reactor neutrino flux motivates revisiting the underlying beta spectra measurements. A method is proposed to use an accelerator proton beam delivered to an engineered target to yield a neutron field tailored to reproduce the neutron energy spectrum present in the core of an operating nuclear reactor. Foils of the primary reactor fissionable isotopes placed in this tailored neutron flux will ultimately emit beta particles from the resultant fission products. Measurement of these beta particles in a time projection chamber with a perpendicular magnetic field provides a distinctive set of systematic considerations for comparison to the original seminal beta spectra measurements. Ancillary measurements such as gamma ray emission and post irradiation radiochemical analysis will further constrain the absolute normalization of beta emissions per fission. The requirements for unfolding the beta spectra measured with this method into a predicted reactor neutrino spectrum are explored. (C) 2015 Published by Elsevier B.V. C1 [Asner, D. M.; Burns, K.; Campbell, L. W.; Greenfield, B.; Kos, M. S.; Orrell, J. L.; Schram, M.; VanDevender, B.; Wood, L. S.; Wootan, D. W.] Pacific Northwest Lab, Richland, WA 99352 USA. RP Kos, MS (reprint author), Pacific Northwest Lab, Richland, WA 99352 USA. EM markskos@gmail.com RI Orrell, John/E-9313-2015 OI Orrell, John/0000-0001-7968-4051 FU U.S. Department of Energy [DE-AC05-76RL01830] FX The research described in this paper was conducted under the Laboratory Directed Research and Development Program at Pacific Northwest National Laboratoiy, a multiprogram national laboratory operated by Battelle for the U.S. Department of Energy under Contract DE-AC05-76RL01830. Detector simulations in this publication were based, in part, on the NIFFTE Fission Time Projection Chamber, and the authors would like to thank the NIFFTE Collaboration for use of their code. NR 20 TC 0 Z9 0 U1 0 U2 6 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD MAR 11 PY 2015 VL 776 BP 75 EP 82 DI 10.1016/j.nima.2014.09.076 PG 8 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA CB2OY UT WOS:000349468500011 ER PT J AU Bazavov, A Karsch, F Maezawa, Y Mukherjee, S Petreczky, P AF Bazavov, A. Karsch, F. Maezawa, Y. Mukherjee, Swagato Petreczky, P. TI In-medium modifications of open and hidden strange-charm mesons from spatial correlation functions SO PHYSICAL REVIEW D LA English DT Article ID SPECTRAL FUNCTIONS; FINITE-TEMPERATURE; HADRONIC SPECTRUM; PHASE-TRANSITION; QUARK PLASMA; LATTICE QCD AB We calculate spatial correlation functions of in-medium mesons consisting of strange-antistrange, strange-anticharm and charm-anticharm quarks in (2 + 1)-flavor lattice QCD using the highly improved staggered quark action. A comparative study of the in-medium modifications of mesons with different flavor contents is performed. We observe significant in-medium modifications for the phi and D-s meson channels already at temperatures around the chiral crossover region. On the other hand, for the J/psi and eta(c) meson channels in-medium modifications remain relatively small around the chiral crossover region and become significant only above 1.3 times the chiral crossover temperature. C1 [Bazavov, A.] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52240 USA. [Karsch, F.; Maezawa, Y.] Univ Bielefeld, Fak Phys, D-33615 Bielefeld, Germany. [Karsch, F.; Mukherjee, Swagato; Petreczky, P.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. RP Bazavov, A (reprint author), Univ Iowa, Dept Phys & Astron, Iowa City, IA 52240 USA. OI Mukherjee, Swagato/0000-0002-3824-1008 FU U.S. Department of Energy [DE-AC02-98CH10886]; Bundesministerium fur Bildung und Forschung [05P12PBCTA]; EU Integrated Infrastructure Initiative Hadron-Physics3; Scientific Discovery through the Advanced Computing (SciDAC) FX Numerical calculations were carried out on the USQCD Clusters at the Jefferson Laboratory, USA, the NYBlue supercomputer at the Brookhaven National Laboratory, USA and in NERSC, USA. This work was partly supported through Contract No. DE-AC02-98CH10886 from the U.S. Department of Energy and the Bundesministerium fur Bildung und Forschung under Grant No. 05P12PBCTA and the EU Integrated Infrastructure Initiative Hadron-Physics3. Partial support for this work was also provided by Scientific Discovery through the Advanced Computing (SciDAC) program funded by the U.S. Department of Energy, Office of Science, Advanced Scientific Computing Research (and Basic Energy Sciences/Biological and Environmental Research/High Energy Physics/Fusion Energy Sciences/Nuclear Physics). The calculations reported in this paper have been performed using the public MILC code (MILC Collaboration: http://www.physics.utah.edu/similar to detar/milc). NR 45 TC 8 Z9 8 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD MAR 10 PY 2015 VL 91 IS 5 AR 054503 DI 10.1103/PhysRevD.91.054503 PG 16 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CE7MM UT WOS:000352025200008 ER PT J AU Calore, F Cholis, I McCabe, C Weniger, C AF Calore, Francesca Cholis, Ilias McCabe, Christopher Weniger, Christoph TI A tale of tails: Dark matter interpretations of the Fermi GeV excess in light of background model systematics SO PHYSICAL REVIEW D LA English DT Article ID GAMMA-RAY EMISSION; GALACTIC-CENTER; CONSTRAINTS; SCALAR; ANNIHILATION; CANDIDATES; REGION AB Several groups have identified an extended excess of gamma rays over the modeled foreground and background emissions towards the Galactic center (GC) based on observations with the Fermi Large Area Telescope. This excess emission is compatible in morphology and spectrum with a telltale sign from dark matter (DM) annihilation. Here, we present a critical reassessment of DM interpretations of the GC signal in light of the foreground and background uncertainties that some of us recently outlaid in Calore et al. (2014). We find that a much larger number of DM models fits the gamma-ray data than previously noted. In particular: (1) In the case of DM annihilation into (b) over barb, we find that even large DM masses up to m(chi) similar or equal to 74 GeV are allowed at p-value > 0.05. (2) Surprisingly, annihilation into nonrelativistic hh gives a good fit to the data. (3) The inverse Compton emission from mu(+)mu(-) with m(chi) similar to 60-70 GeV can also account for the excess at higher latitudes, vertical bar b vertical bar > 2 degrees, both in its spectrum and morphology. We also present novel constraints on a large number of mixed annihilation channels, including cascade annihilation involving hidden sector mediators. Finally, we show that the current limits from dwarf spheroidal observations are not in tension with a DM interpretation when uncertainties on the DM halo profile are accounted for. C1 [Calore, Francesca; McCabe, Christopher; Weniger, Christoph] Univ Amsterdam, GRAPPA, NL-1098 XH Amsterdam, Netherlands. [Cholis, Ilias] Fermilab Natl Accelerator Lab, Ctr Particle Astrophys, Batavia, IL 60510 USA. RP Calore, F (reprint author), Univ Amsterdam, GRAPPA, Sci Pk 904, NL-1098 XH Amsterdam, Netherlands. EM f.calore@uva.nl; cholis@fnal.gov; c.mccabe@uva.nl; c.weniger@uva.nl FU Netherlands Organisation for Scientific Research (NWO); U.S. Department of Energy; European Research Council through the ERC FX We thank Markus Ackermann, Carmelo Evoli, Dan Hooper, Gudlaugur Johannesson, Simona Murgia, Troy Porter and Neal Weiner for useful discussions. The research of C. W. is part of the VIDI research programme "Probing the Genesis of Dark Matter," which is financed by the Netherlands Organisation for Scientific Research (NWO). This work has been supported by the U.S. Department of Energy. F. C. and C. M. acknowledge support from the European Research Council through the ERC starting grant WIMPs Kairos, principal investigator G. Bertone. NR 127 TC 97 Z9 97 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 10 PY 2015 VL 91 IS 6 AR 063003 DI 10.1103/PhysRevD.91.063003 PG 18 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CE7MQ UT WOS:000352025900002 ER PT J AU Christ, NH Flynn, JM Izubuchi, T Kawanai, T Lehner, C Soni, A Van de Water, RS Witzel, O AF Christ, N. H. Flynn, J. M. Izubuchi, T. Kawanai, T. Lehner, C. Soni, A. Van de Water, R. S. Witzel, O. CA RBC Collaboration UKQCD Collaboration TI B-meson decay constants from 2+1-flavor lattice QCD with domain-wall light quarks and relativistic heavy quarks SO PHYSICAL REVIEW D LA English DT Article ID CHIRAL FERMIONS AB We calculate the B-meson decay constants f(B), f(Bs), and their ratio in unquenched lattice QCD using domain-wall light quarks and relativistic b quarks. We use gauge-field ensembles generated by the RBC and UKQCD collaborations using the domain-wall fermion action and Iwasaki gauge action with three flavors of light dynamical quarks. We analyze data at two lattice spacings of a approximate to 0.11, 0.086 fm with unitary pion masses as light as M-pi approximate to 290 MeV; this enables us to control the extrapolation to the physical light-quark masses and continuum. For the b quarks we use the anisotropic clover action with the relativistic heavy-quark interpretation, such that discretization errors from the heavy-quark action are of the same size as from the light-quark sector. We renormalize the lattice heavy-light axial-vector current using a mostly nonperturbative method in which we compute the bulk of the matching factor nonperturbatively, with a small correction, that is close to unity, in lattice perturbation theory. We also improve the lattice heavy-light current through O(alpha(s)a). We extrapolate our results to the physical light-quark masses and continuum using SU(2) heavy-meson chiral perturbation theory, and provide a complete systematic error budget. We obtain f(B0) = 199.5(12.6) MeV, f(B+) = 195.6(14.9) MeV, f(Bs) = 235.4(12.2) MeV, f(Bs)/f(B0) = 1.197(50), and f(Bs)/f(B+) = 1.223(71), where the errors are statistical and total systematic added in quadrature. These results are in good agreement with other published results and provide an important independent cross-check of other three-flavor determinations of B-meson decay constants using staggered light quarks. C1 [Christ, N. H.] Columbia Univ, Dept Phys, New York, NY 10027 USA. [Flynn, J. M.] Univ Southampton, Sch Phys & Astron, Southampton SO17 1BJ, Hants, England. [Izubuchi, T.] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. [Izubuchi, T.; Kawanai, T.; Lehner, C.; Soni, A.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Kawanai, T.] RIKEN, Nishina Ctr, Theoret Res Div, Wako, Saitama 3510198, Japan. [Van de Water, R. S.] Fermilab Natl Accelerator Lab, Dept Theoret Phys, Batavia, IL 60510 USA. [Witzel, O.] Boston Univ, Ctr Computat Sci, Boston, MA 02215 USA. RP Christ, NH (reprint author), Columbia Univ, Dept Phys, 538 W 120th St, New York, NY 10027 USA. OI Lehner, Christoph/0000-0002-3584-4567; Flynn, Jonathan/0000-0002-6280-1677 FU Office of Science of the U.S. Department of Energy; U.S. Department of Energy [DE-FG02-92ER40699, DE-AC02-98CH10886]; United Kingdom Science and Technology Facilities Council (STFC) Grant [ST/J000396/1]; Ministry of Education, Culture, Sports, Science and Technology, Japan (MEXT) [26400261, 22540301, 23105715]; JSPS [R2411]; Boston University by the U.S. DOE [DE-SC0008814] FX Computations for this work were carried out in part on facilities of the USQCD Collaboration, which are funded by the Office of Science of the U.S. Department of Energy. We thank BNL, Columbia University, Fermilab, RIKEN, and the U.S. DOE for providing the facilities essential for the completion of this work.; This work was supported in part by the U.S. Department of Energy under Award No. DE-FG02-92ER40699 (N. H. C.), by the United Kingdom Science and Technology Facilities Council (STFC) Grant No. ST/J000396/1 (J. M. F.), and by the Grant-in-Aid of the Ministry of Education, Culture, Sports, Science and Technology, Japan (MEXT) Grants No. 26400261, No. 22540301, and No. 23105715 (T. I). T. K. is supported by the JSPS Strategic Young Researcher Overseas Visits Program for Accelerating Brain Circulation (Grant No. R2411). O. W. acknowledges support at Boston University by the U.S. DOE Award No. DE-SC0008814. This manuscript has been authored by employees of Brookhaven Science Associates, LLC, under Contract No. DE-AC02-98CH10886 with the U.S. Department of Energy. NR 57 TC 16 Z9 16 U1 1 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 10 PY 2015 VL 91 IS 5 AR 054502 DI 10.1103/PhysRevD.91.054502 PG 24 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CE7MM UT WOS:000352025200007 ER PT J AU Wilson, DJ Dudek, JJ Edwards, RG Thomas, CE AF Wilson, David J. Dudek, Jozef J. Edwards, Robert G. Thomas, Christopher E. CA Hadron Spectrum Collaboration TI Resonances in coupled pi K,eta K scattering from lattice QCD SO PHYSICAL REVIEW D LA English DT Article ID PI-K SCATTERING; FINITE-VOLUME; VECTOR-MESONS; PHASE-SHIFTS; 11 GEV/C; STATES; PARTICLES; SYSTEMS; MATRIX; DECAYS AB Coupled-channel pi K and eta K scattering amplitudes are determined by studying the finite-volume energy spectra obtained from dynamical lattice QCD calculations. Using a large basis of interpolating operators, including both those resembling a q (q) over barq construction and those resembling a pair of mesons with relative momentum, a reliable excited-state spectrum can be obtained. Working at m(pi) = 391 MeV, we find a gradual increase in the J(P) =0(+) pi K phase shift which may be identified with a broad scalar resonance that couples strongly to pi K and weakly to eta K. The low-energy behavior of this amplitude suggests a virtual bound state that may be related to the. resonance. A bound state with J(P) = 1(-) is found very close to the pi K threshold energy, whose coupling to the pi K channel is compatible with that of the experimental K star(892). Evidence is found for a narrow resonance in J(P) = 2(+). Isospin-3/2 pi K scattering is also studied, and nonresonant phase shifts spanning the whole elastic scattering region are obtained. C1 [Wilson, David J.; Dudek, Jozef J.] Old Dominion Univ, Dept Phys, Norfolk, VA 23529 USA. [Dudek, Jozef J.; Edwards, Robert G.] Ctr Theory, Jefferson Lab, Newport News, VA 23606 USA. [Thomas, Christopher E.] Univ Cambridge, Ctr Math Sci, Dept Appl Math & Theoret Phys, Cambridge CB3 0WA, England. RP Wilson, DJ (reprint author), Old Dominion Univ, Dept Phys, Norfolk, VA 23529 USA. EM dudek@jlab.org FU U.S. Department of Energy INCITE program at Oak Ridge National Lab; NSF Teragrid at the Texas Advanced Computer Center; Pittsburgh Supercomputer Center; Jefferson Lab; U.S. Department of Energy [DE-AC05-06OR23177]; U.S. Department of Energy Early Career award [DE-SC0006765]; Science and Technology Facilities Council (UK) [ST/L000385/1] FX We thank our colleagues within the Hadron Spectrum Collaboration. We also thank R. Briceno, M. R. Pennington, C. J. Shultz, and A. P. Szczepaniak for fruitfuldiscussions. CHROMA [63] and QUDA [64,65] were used to perform this work on clusters at Jefferson Laboratory under the USQCD Initiative and the LQCD ARRA project. Gauge configurations were generated using resources awarded from the U.S. Department of Energy INCITE program at Oak Ridge National Lab, the NSF Teragrid at the Texas Advanced Computer Center, and the Pittsburgh Supercomputer Center, as well as at Jefferson Lab. R. G. E. and J. J. D. acknowledge support from U.S. Department of Energy Contract No. DE-AC05-06OR23177, under which Jefferson Science Associates, LLC, manages and operates Jefferson Laboratory. J. J. D. acknowledges support from the U.S. Department of Energy Early Career award Contract No. DE-SC0006765. C. E. T. acknowledges partial support from the Science and Technology Facilities Council (UK) (Grant No. ST/L000385/1). NR 66 TC 30 Z9 30 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD MAR 10 PY 2015 VL 91 IS 5 AR 054008 DI 10.1103/PhysRevD.91.054008 PG 34 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CE7MM UT WOS:000352025200002 ER PT J AU Kagan, AL Perez, G Petriello, F Soreq, Y Stoynev, S Zupan, J AF Kagan, Alexander L. Perez, Gilad Petriello, Frank Soreq, Yotam Stoynev, Stoyan Zupan, Jure TI Exclusive Window onto Higgs Yukawa Couplings SO PHYSICAL REVIEW LETTERS LA English DT Article ID MESON DISTRIBUTION AMPLITUDE; ATLAS DETECTOR; FINAL-STATES; BOSON; LHC; PARTICLE; DECAYS; DISTRIBUTIONS; PHYSICS; QCD AB We show that both flavor-conserving and flavor-violating Yukawa couplings of the Higgs boson to first- and second-generation quarks can be probed by measuring rare decays of the form h --> MV, where M denotes a vector meson and V indicates either gamma, W or Z. We calculate the branching ratios for these processes in both the standard model and its possible extensions. We discuss the experimental prospects for their observation. The possibility of accessing these Higgs couplings appears to be unique to the high-luminosity LHC and future hadron colliders, providing further motivation for those machines. C1 [Kagan, Alexander L.; Zupan, Jure] Univ Cincinnati, Dept Phys, Cincinnati, OH 45221 USA. [Perez, Gilad] CERN, Div Theory, CH-1211 Geneva 23, Switzerland. [Perez, Gilad; Soreq, Yotam] Weizmann Inst Sci, Dept Particle Phys & Astrophys, IL-7610001 Rehovot, Israel. [Petriello, Frank] Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. [Petriello, Frank; Stoynev, Stoyan] Northwestern Univ, Dept Phys & Astron, Evanston, IL 60208 USA. RP Kagan, AL (reprint author), Univ Cincinnati, Dept Phys, Cincinnati, OH 45221 USA. EM kaganal@ucmail.uc.edu; gilad.perez@cern.ch; f-petriello@northwestern.edu; yotam.soreq@weizmann.ac.il; stoyan.stoynev@cern.ch; zupanje@ucmail.uc.edu FU DOE [DE-SC0011784, DE-FG02-91ER40684, DE-AC02-06CH11357]; Minerva foundation; IRG; ERC; Gruber award; U.S. National Science Foundation under CAREER Grant [PHY-1151392] FX We thank the CERN theory group, where this work was initiated, for its hospitality. A. L. K. and J. Z. thank M. Neubert, and F. P. thanks K. Mishra for discussions. The work of A. L. K. is supported by DOE Grant No. DE-SC0011784. G. P. is supported by the Minerva foundation, the IRG, ERC, and by the Gruber award. F. P. is supported by DOE Grants No. DE-FG02-91ER40684 and No. DE-AC02-06CH11357. S. S. is supported by DOE Grant No. DE-FG02-91ER40684. J. Z. is supported in part by the U.S. National Science Foundation under CAREER Grant No. PHY-1151392. NR 60 TC 28 Z9 28 U1 1 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 10 PY 2015 VL 114 IS 10 AR 101802 DI 10.1103/PhysRevLett.114.101802 PG 5 WC Physics, Multidisciplinary SC Physics GA CE8EE UT WOS:000352073400008 PM 25815924 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schofbeck, R Strauss, J Taurok, A Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, M Bansal, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Luyckx, S Ochesanu, S Rougny, R De Klundert, MV Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Daci, N Heracleous, N Keaveney, J Lowette, S Maes, M Olbrechts, A Python, Q Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Caillol, C Clerbaux, B De Lentdecker, G Dobur, D Favart, L Gay, APR Grebenyuk, A Leonard, A Mohammadi, A Pernie, L Reis, T Seva, T Thomas, L Velde, CV Vanlaer, P Wang, J Zenoni, F Adler, V Beernaert, K Benucci, L Cimmino, A Costantini, S Crucy, S Dildick, S Fagot, A Garcia, G Mccartin, J Rios, AAO Ryckbosch, D Diblen, SS Sigamani, M Strobbe, N Thyssen, F Tytgat, M Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bruno, G Castello, R Caudron, A Ceard, L Da Silveira, GG Delaere, C du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Jafari, A Jez, P Komm, M Lemaitre, V Nuttens, C Pagano, D Perrini, L Pin, A Piotrzkowski, K Popov, A Quertenmont, L Selvaggi, M Marono, MV Garcia, JMV Beliy, N Caebergs, T Daubie, E Hammad, GH Alda, WL Alves, GA Brito, L Martins, M Martins, TD Herrera, CM Pol, ME Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD De Souza, SF Malbouisson, H Figueiredo, D Mundim, L Nogima, H Da Silva, WLP Santaolalla, J Santoro, A Sznajder, A Manganote, EJT Pereira, AV Bernardes, CA Dogra, S Tomei, TRFP Gregores, EM Mercadante, PG Novaes, SF Padula, S Aleksandrov, A Genchev, V Iaydjiev, P Marinov, A Piperov, S Rodozov, M Stoykova, S Sultanov, G Tcholakov, V Vutova, M Dimitrov, A Glushkov, I Hadjiiska, R Kozhuharov, V Litov, L Pavlov, B Petkov, P Bian, JG Chen, GM Chen, HS Chen, M Du, R Jiang, CH Plestina, R Tao, J Wang, Z Asawatangtrakuldee, C Ban, Y Li, Q Liu, S Mao, Y Qian, SJ Wang, D Zhang, L Avila, C Sierra, LFC Florez, C Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Polic, D Puljak, I Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Mekterovic, D Sudic, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Bodlak, M Finger, M Finger, M Assran, Y Kamel, AE Mahmoud, MA Radi, A Kadastik, M Murumaa, M Raidal, M Tiko, A Eerola, P Fedi, G Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Kortelainen, MJ Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E Wendland, L Talvitie, J Tuuva, T Besancon, M Couderc, F Dejardin, M Denegri, D Fabbro, B Faure, JL Favaro, C Ferri, F Ganjour, S Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Malcles, J Rander, J Rosowsky, A Titov, M Baffioni, S Beaudette, F Busson, P Charlot, C Dahms, T Dalchenko, M Dobrzynski, L Filipovic, N Florent, A de Cassagnac, RG Mastrolorenzo, L Mine, P Mironov, C Naranjo, IN Nguyen, M Ochando, C Paganini, P Regnard, S Salerno, R Sauvan, JB Sirois, Y Veelken, C Yilmaz, Y Zabi, A Agram, JL Andrea, J Aubin, A Bloch, D Brom, JM Chabert, EC Collard, C Conte, E Fontaine, JC Fuks, B Gele, D Goerlach, U Goetzmann, C Le Bihan, AC Van Hove, P Gadrat, S Beauceron, S Beaupere, N Boudoul, G Bouvier, E Brochet, S Montoya, CAC Chasserat, J Chierici, R Contardo, D Depasse, P El Mamouni, H Fan, J Fay, J Gascon, S Gouzevitch, M Ille, B Kurca, T Lethuillier, M Mirabito, L Perries, S Alvarez, JDR Sabes, D Sgandurra, L Sordini, V Donckt, MV Verdier, P Viret, S Xiao, H Rurua, L Autermann, C Beranek, S 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Hall-Wilton, R. Herndon, M. Herve, A. Klabbers, P. Lanaro, A. Lazaridis, C. Levine, A. Loveless, R. Mohapatra, A. Ojalvo, I. Perry, T. Pierro, G. A. Polese, G. Ross, I. Sarangi, T. Savin, A. Smith, W. H. Taylor, D. Verwilligen, P. Vuosalo, C. Woods, N. CA CMS Collaboration TI Search for Monotop Signatures in Proton-Proton Collisions at root s=8 TeV SO PHYSICAL REVIEW LETTERS LA English DT Article ID SUPERSYMMETRY; PHYSICS AB Results are presented from a search for new decaying massive particles whose presence is inferred from an imbalance in transverse momentum and which are produced in association with a single top quark that decays into a bottom quark and two light quarks. The measurement is performed using 19.7 fb(-1) of data from proton-proton collisions at a center-of-mass energy of 8 TeV, collected with the CMS detector at the CERN LHC. No deviations from the standard model predictions are observed and lower limits are set on the masses of new invisible bosons. In particular, scalar and vector particles, with masses below 330 and 650 GeV, respectively, are excluded at 95% confidence level, thereby substantially extending a previous limit published by the CDF Collaboration. C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Bergauer, T.; Dragicevic, M.; Eroe, J.; Fabjan, C.; Friedl, M.; Fruehwirth, R.; Ghete, V. M.; Hartl, C.; Hoermann, N.; Jeitler, M.; Kiesenhofer, W.; Knuenz, V.; Krammer, M.; Liko, D.; Mikulec, I.; Rabady, D.; Rahbaran, B.; Rohringer, H.; Schoefbeck, R.; Taurok, A.; Treberer-Treberspurg, W.; Waltenberger, W.; Wulz, C. -E.] Inst Hochenergiephys OeAW, Vienna, Austria. [Mossolov, V.; Shumeiko, N.; Gonzalez, J. Suarez] Natl Ctr Particle & High Energy Phys, Minsk, Byelarus. [Alderweireldt, S.; Bansal, M.; Bansal, S.; Cornelis, T.; De Wolf, E. A.; Janssen, X.; Knutsson, A.; Ochesanu, S.; Rougny, R.; De Klundert, M. 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M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.; Umer, T.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.; Umer, T.] Univ Trieste, Trieste, Italy. [Chang, S.; Kropivnitskaya, A.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Park, H.; Sakharov, A.; Son, D. C.] Kyungpook Natl Univ, Daegu, South Korea. [Kim, T. J.] Chonbuk Natl Univ, Jeonju 561756, South Korea. [Kim, J. Y.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, Y.; Lee, B.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, I. C.; Ryu, G.; Ryu, M. S.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, D.; Kwon, E.; Lee, J.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.] Vilnius State Univ, Vilnius, Lithuania. [Komaragiri, J. R.; Ali, M. A. B. Md] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Castilla-Valdez, H.; De la Cruz-Burelo, E.; Heredia-de la Cruz, I.; Hernandez-Almada, A.; Lopez-Fernandez, R.; Sanchez-Hernandez, A.] Ctr Invest & Estudios Avanzados IPN, Mexico City, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Pedraza, I.; Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Reucroft, S.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, A.; Ahmad, M.; Hassan, Q.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.; Wolszczak, W.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz E Silva, C.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Lloret Iglesias, L.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Finger, M., Jr.; Bunin, P.; Golutvin, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Kozlov, G.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Savina, M.; Shmatov, S.; Shulha, S.; Skatchkov, N.; Smirnov, V.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Matveev, V.; Andreev, Yu.; Dermenev, A.; Gninenko, S.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Popov, A.; Zhukov, V.; Katkov, I.; Belyaev, A.; Boos, E.; Bunichev, V.; Dubinin, M.; Dudko, L.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Obraztsov, S.; Perfilov, M.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Volkov, A.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia. [Adzic, P.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.; Sphicas, P.; Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.; Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Alcaraz Maestre, J.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De la Cruz, B.; Delgado Peris, A.; Domnguez Vazquez, D.; Escalante Del Valle, A.; Bedoya, C. Fernandez; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.] CIEMAT, Ctr Invest Energet Medioambientales & Tecnol, E-28040 Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.] Univ Oviedo, Oviedo, Spain. [Rodrigues Antunes, J.; Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Graziano, A.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Rabady, D.; Pernie, L.; Genchev, V.; Bloch, D.; Boudoul, G.; Contardo, D.; Lingemann, J.; Hartmann, F.; Hauth, T.; Kornmayer, A.; Mohanty, A. K.; Radogna, R.; Silvestris, L.; Giordano, F.; Gori, V.; Fiorendi, S.; Gerosa, R.; Lucchini, M. T.; Di Guida, S.; Meola, S.; Paolucci, P.; Spiezia, A.; Palla, F.; Vernieri, C.; Micheli, F.; Soffi, L.; Argiro, S.; Obertino, M. M.; Casarsa, M.; Schizzi, A.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; David, A.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Franzoni, G.; Funk, W.; Gigi, D.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Hansen, M.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Magini, N.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Musella, P.; Orsini, L.; Pape, L.; Perrozzi, L.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Piparo, D.; Plagge, M.; Racz, A.; Rovere, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Steggemann, J.; Stieger, B.; Stoye, M.; Takahashi, Y.; Treille, D.; Tsirou, A.; Veres, G. 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Millan; Ngadiuba, J.; Robmann, P.; Ronga, F. J.; Taroni, S.; Verzetti, M.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Lu, Y. J.; Volpe, R.; Yu, S. S.; Lin, C.] Natl Cent Univ, Chungli 32054, Taiwan. [Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Grundler, U.; Hou, W. -S.; Kao, K. Y.; Lei, Y. J.; Liu, Y. F.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Tzeng, Y. M.; Wilken, R.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Fac Sci, Dept Phys, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Gamsizkan, H.; Karapinar, G.; Ocalan, K.; Sekmen, S.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.] Bogazici Univ, Istanbul, Turkey. [Cankocak, K.; Vardarli, F. I.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Ctr Nat Sci, Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Belyaev, A.; Newbold, D. M.; Bell, K. W.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Womersley, W. J.; Worm, S. D.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Dunne, P.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Hall, G.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Mathias, B.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Lawson, P.; Richardson, C.; Rohlf, J.; St John, J.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Naranjo, I. N.; Bhattacharya, S.; Alimena, J.; Berry, E.; Christopher, G.; Cutts, D.; Demiragli, Z.; Dhingra, N.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Segala, M.; Sinthuprasith, T.; Speer, T.; Swanson, J.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Lander, R.; Miceli, T.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Searle, M.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.; Cox, B.] Univ Calif Davis, Davis, CA 95616 USA. [Weber, M.; Cousins, R.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Rakness, G.; Takasugi, E.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Rikova, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Nguyen, H.; Negrete, M. Olmedo; Shrinivas, A.; Sumowidagdo, S.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sharma, V.; Simon, M.; Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Evans, D.; Holzner, A.; Kelley, R.; Klein, D.; Lebourgeois, M.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Palmer, C.; Pieri, M.; Sani, M.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Welke, C.; Wuerthwein, F.; Yagil, A.] Univ Calif San Diego, San Diego, CA 92103 USA. [Barge, D.; Bradmiller-Feld, J.; Campagnari, C.; Danielson, T.; Dishaw, A.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Incandela, J.; Justus, C.; Richman, J.; Stuart, D.; To, W.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dubinin, M.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Wilkinson, R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Iiyama, Y.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Skinnari, L.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Kaadze, K.; Klima, B.; Kwan, S.; Lincoln, D.; Lipton, R.; Liu, T.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Sexton-Kennedy, E.; Sharma, S.; Soha, A.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Yang, F.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Carver, M.; Cheng, T.; Curry, D.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Field, R. D.; Fisher, M.; Furic, I. K.; Hugon, J.; Konigsberg, J.; Korytov, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Rinkevicius, A.; Shchutska, L.; Snowball, M.; Sperka, D.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Moon, C. S.; Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; O'Brien, C.; Silkworth, C.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Haytmyradov, M.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Rahmat, R.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Swartz, M.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Bruner, C.; Kenny, R. P., III; Malek, M.; Murray, M.; Noonan, D.; Sanders, S.; Sekaric, J.; Stringer, R.; Wang, Q.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Belloni, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Bauer, G.; Busza, W.; Cali, I. A.; Chan, M.; Di Matteo, L.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Klute, M.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Ma, T.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Velicanu, D.; Veverka, J.; Wyslouch, B.; Yang, M.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; Gude, A.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, Oxford, MS USA. [Malik, S.; Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Suarez, R. Gonzalez; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Meier, F.; Zvada, M.] Univ Nebraska, Lincoln, NE USA. [Kumar, A.; Dolen, J.; Godshalk, A.; Iashvili, I.; Kharchilava, A.; Rappoccio, S.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; Trocino, D.; Wang, R. -J.; Wood, D.; Zhang, J.] Northwestern Univ, Boston, MA USA. [Hahn, K. A.; Kubik, A.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Velasco, M.] Northwestern Univ, Evanston, IL USA. [Brinkerhoff, A.; Chan, K. M.; Drozdetskiy, A.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Pearson, T.; Planer, M.; Ruchti, R.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Puigh, D.; Rodenburg, M.; Smith, G.; Winer, B. L.; Wolfe, H.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Driga, O.; Elmer, P.; Hebda, P.; Hunt, A.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Brownson, E.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA. [Savoy-Navarro, A.; Barnes, V. E.; Benedetti, D.; Bortoletto, D.; De Mattia, M.; Gutay, L.; Hu, Z.; Jha, M. K.; Jones, M.; Jung, K.; Kress, M.; Leonardo, N.; Pegna, D. Lopes; Maroussov, V.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shi, X.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.; Stupak, J.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Ecklund, K. M.; Geurts, F. J. M.; Li, W.; Michlin, B.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; Covarelli, R.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Khukhunaishvili, A.; Petrillo, G.; Vishnevskiy, D.] Univ Rochester, Rochester, NY USA. [Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Kaplan, S.; Lath, A.; Panwalkar, S.; Park, M.; Patel, R.; Salur, S.; Schnetzer, S.; Somalwar, S.; Stone, R.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Rose, K.; Spanier, S.; York, A.] Univ Tennessee, Knoxville, TN USA. [Rose, A.; Bouhali, O.; Hernandez, A. Castaneda; Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Khotilovich, V.; Krutelyov, V.; Montalvo, R.; Osipenkov, I.; Pakhotin, Y.; Perloff, A.; Roe, J.; Safonov, A.; Sakuma, T.; Suarez, I.; Tatarinov, A.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kovitanggoon, K.; Kunori, S.; Lee, S. W.; Libeiro, T.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Mao, Y.; Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Johns, W.; Maguire, C.; Melo, A.; Sharma, M.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN 37235 USA. [Arenton, M. W.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Li, H.; Lin, C.; Neu, C.; Wood, J.] Univ Virginia, Charlottesville, VA USA. [Clarke, C.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sturdy, J.] Wayne State Univ, Detroit, MI USA. [Belknap, D. A.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Dodd, L.; Duric, S.; Friis, E.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Lanaro, A.; Lazaridis, C.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Ross, I.; Sarangi, T.; Savin, A.; Smith, W. H.; Taylor, D.; Verwilligen, P.; Vuosalo, C.; Woods, N.] Univ Wisconsin, Madison, WI USA. [Sharp, P.] Vienna Univ Technol, A-1040 Vienna, Austria. [Chinellato, J.; Tonelli Manganote, E. J.] Univ Estadual Campinas, Campinas, SP, Brazil. [Assran, Y.] Suez Univ, Suez, Egypt. [Kamel, A. Ellithi] Cairo Univ, Cairo, Egypt. [Mahmoud, M. A.] Fayoum Univ, Al Fayyum, Egypt. [Radi, A.] British Univ Egypt, Cairo, Egypt. [Radi, A.] Ain Shams Univ, Cairo, Egypt. [Agram, J. -L.; Conte, E.; Fontaine, J. -C.] Univ Haute Alsace, Mulhouse, France. [Bergholz, M.; Hempel, M.; Lohmann, W.; Marfin, I.; Schmidt, R.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Vesztergombi, G.; Bhowmik, S.; Veres, G. I.] Eotvos Lorand Univ, Budapest, Hungary. [Bhowmik, S.; Maity, M.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Gurtu, A.] King Abdulaziz Univ, Jeddah 21413, Saudi Arabia. [Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka. [Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Fahim, A.] Sharif Univ Technol, Tehran, Iran. [Safarzadeh, B.] Islamic Azad Univ, Sci & Res Branch, Plasma Phys Res Ctr, Tehran, Iran. [Androsov, K.; Ciocci, M. A.; Grippo, M. T.; Squillacioti, P.] Univ Siena, I-53100 Siena, Italy. [Moon, C. S.] CNRS, IN2P3, Paris, France. [Heredia-de la Cruz, I.] Univ Michoacana, Morelia, Michoacan, Mexico. [Kim, V.] St Petersburg State Polytech Univ, St Petersburg, Russia. [Colafranceschi, S.] Univ Roma La Sapienza, Fac Ingn, I-00185 Rome, Italy. [Rolandi, G.] Scuola Normale & Sez INFN, Pisa, Italy. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Bakirci, M. N.; Ozturk, S.; Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey. [Cerci, S.; Cerci, D. Sunar; Tali, B.] Adiyaman Univ, Adiyaman, Turkey. [Onengut, G.] Cag Univ, Mersin, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Ocalan, K.] Necmettin Erbakan Univ, Konya, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Kaya, M.] Marmara Univ, Istanbul, Turkey. [Kaya, O.] Kafkas Univ, Kars, Turkey. [Belyaev, A.] Kafkas Univ, Kars, Turkey. [Albayrak, E. A.; Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Bilki, B.] Argonne Natl Lab, Argonne, IL 60439 USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Yetkin, T.] Yildiz Tekn Univ, Istanbul, Turkey. [Bouhali, O.] Texas A&M Univ Qatar, Doha, Qatar. RP Khachatryan, V (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Menasce, Dario Livio/A-2168-2016; Rolandi, Luigi (Gigi)/E-8563-2013; Sguazzoni, Giacomo/J-4620-2015; Ligabue, Franco/F-3432-2014; Goh, Junghwan/Q-3720-2016; Ruiz, Alberto/E-4473-2011; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Paulini, Manfred/N-7794-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Ogul, Hasan/S-7951-2016; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Da Silveira, Gustavo Gil/N-7279-2014; Mora Herrera, Maria Clemencia/L-3893-2016; Mundim, Luiz/A-1291-2012; Haj Ahmad, Wael/E-6738-2016; Konecki, Marcin/G-4164-2015; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Calderon, Alicia/K-3658-2014; Manganote, Edmilson/K-8251-2013; Cavallo, Nicola/F-8913-2012; Montanari, Alessandro/J-2420-2012; Lokhtin, Igor/D-7004-2012; Hernandez Calama, Jose Maria/H-9127-2015; VARDARLI, Fuat Ilkehan/B-6360-2013; Sen, Sercan/C-6473-2014; D'Alessandro, Raffaello/F-5897-2015; Wulz, Claudia-Elisabeth/H-5657-2011; Belyaev, Alexander/F-6637-2015; Stahl, Achim/E-8846-2011; Trocsanyi, Zoltan/A-5598-2009; Cerrada, Marcos/J-6934-2014; Perez-Calero Yzquierdo, Antonio/F-2235-2013; Novaes, Sergio/D-3532-2012; Della Ricca, Giuseppe/B-6826-2013; Chinellato, Jose Augusto/I-7972-2012; Tomei, Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Tinoco Mendes, Andre David/D-4314-2011; Seixas, Joao/F-5441-2013; Andreev, Vladimir/M-8665-2015; Cakir, Altan/P-1024-2015; Matorras, Francisco/I-4983-2015; Gennai, Simone/P-2880-2015; TUVE', Cristina/P-3933-2015; Dudko, Lev/D-7127-2012; KIM, Tae Jeong/P-7848-2015; Paganoni, Marco/A-4235-2016; Azarkin, Maxim/N-2578-2015; de Jesus Damiao, Dilson/G-6218-2012; Horani, Hafeez /L-2414-2015; Calvo Alamillo, Enrique/L-1203-2014; Flix, Josep/G-5414-2012; ciocci, maria agnese /I-2153-2015; Bedoya, Cristina/K-8066-2014; My, Salvatore/I-5160-2015; Benussi, Luigi/O-9684-2014; Lo Vetere, Maurizio/J-5049-2012; Ragazzi, Stefano/D-2463-2009; Grandi, Claudio/B-5654-2015; Rovelli, Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Dogra, Sunil /B-5330-2013; Leonidov, Andrey/M-4440-2013 OI Benaglia, Andrea Davide/0000-0003-1124-8450; Covarelli, Roberto/0000-0003-1216-5235; Ciulli, Vitaliano/0000-0003-1947-3396; Androsov, Konstantin/0000-0003-2694-6542; Fiorendi, Sara/0000-0003-3273-9419; Martelli, Arabella/0000-0003-3530-2255; Gonzi, Sandro/0000-0003-4754-645X; Levchenko, Petr/0000-0003-4913-0538; Giubilato, Piero/0000-0003-4358-5355; Gallinaro, Michele/0000-0003-1261-2277; Boccali, Tommaso/0000-0002-9930-9299; Menasce, Dario Livio/0000-0002-9918-1686; Gerosa, Raffaele/0000-0001-8359-3734; Attia Mahmoud, Mohammed/0000-0001-8692-5458; Bilki, Burak/0000-0001-9515-3306; Rolandi, Luigi (Gigi)/0000-0002-0635-274X; Sguazzoni, Giacomo/0000-0002-0791-3350; Casarsa, Massimo/0000-0002-1353-8964; Ligabue, Franco/0000-0002-1549-7107; Diemoz, Marcella/0000-0002-3810-8530; Tricomi, Alessia Rita/0000-0002-5071-5501; Ghezzi, Alessio/0000-0002-8184-7953; Demaria, Natale/0000-0003-0743-9465; Goh, Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787; Ogul, Hasan/0000-0002-5121-2893; Bean, Alice/0000-0001-5967-8674; Longo, Egidio/0000-0001-6238-6787; Di Matteo, Leonardo/0000-0001-6698-1735; Baarmand, Marc/0000-0002-9792-8619; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Mundim, Luiz/0000-0001-9964-7805; Haj Ahmad, Wael/0000-0003-1491-0446; Konecki, Marcin/0000-0001-9482-4841; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Montanari, Alessandro/0000-0003-2748-6373; Hernandez Calama, Jose Maria/0000-0001-6436-7547; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Belyaev, Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279; Cerrada, Marcos/0000-0003-0112-1691; Perez-Calero Yzquierdo, Antonio/0000-0003-3036-7965; Novaes, Sergio/0000-0003-0471-8549; Della Ricca, Giuseppe/0000-0003-2831-6982; Chinellato, Jose Augusto/0000-0002-3240-6270; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Seixas, Joao/0000-0002-7531-0842; Matorras, Francisco/0000-0003-4295-5668; TUVE', Cristina/0000-0003-0739-3153; Dudko, Lev/0000-0002-4462-3192; KIM, Tae Jeong/0000-0001-8336-2434; Paganoni, Marco/0000-0003-2461-275X; de Jesus Damiao, Dilson/0000-0002-3769-1680; Calvo Alamillo, Enrique/0000-0002-1100-2963; Flix, Josep/0000-0003-2688-8047; ciocci, maria agnese /0000-0003-0002-5462; Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680; Benussi, Luigi/0000-0002-2363-8889; Lo Vetere, Maurizio/0000-0002-6520-4480; Ragazzi, Stefano/0000-0001-8219-2074; Grandi, Claudio/0000-0001-5998-3070; Rovelli, Tiziano/0000-0002-9746-4842; FU BMWFW (Austria); FWF (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MES (Bulgaria); CERN; CAS (China); MoST (China); NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); CSF (Croatia); RPF (Cyprus); MoER (Estonia); ERC IUT (Estonia); ERDF (Estonia); Academy of Finland (Finland); MEC (Finland); HIP (Finland); CEA (France); CNRS/IN2P3 (France); BMBF (Germany); DFG (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NIH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF (Republic of Korea); WCU (Republic of Korea); LAS (Lithuania); MOE (Malaysia); UM (Malaysia); CINVESTAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE (Poland); NSC (Poland); FCT (Portugal); JINR (Dubna); MON (Russia); RosAtom (Russia); RAS (Russia); RFBR (Russia); MESTD (Serbia); SEIDI (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter (Thailand); IPST (Thailand); STAR (Thailand); NSTDA (Thailand); TUBITAK (Turkey); TAEK (Turkey); NASU (Ukraine); SFFR (Ukraine); STFC (United Kingdom); DOE (USA); NSF (USA) FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWFW and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES and CSF (Croatia); RPF (Cyprus); MoER, ERC IUT and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NIH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF and WCU (Republic of Korea); LAS (Lithuania); MOE and UM (Malaysia); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Dubna); MON, RosAtom, RAS and RFBR (Russia); MESTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter, IPST, STAR and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU and SFFR (Ukraine); STFC (United Kingdom); DOE and NSF (USA). NR 50 TC 6 Z9 6 U1 9 U2 56 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 10 PY 2015 VL 114 IS 10 AR UNSP 101801 DI 10.1103/PhysRevLett.114.101801 PG 16 WC Physics, Multidisciplinary SC Physics GA CE8EE UT WOS:000352073400007 ER PT J AU Wang, Y Berlijn, T Hirschfeld, PJ Scalapino, DJ Maier, TA AF Wang, Y. Berlijn, T. Hirschfeld, P. J. Scalapino, D. J. Maier, T. A. TI Glide-Plane Symmetry and Superconducting Gap Structure of Iron-Based Superconductors SO PHYSICAL REVIEW LETTERS LA English DT Article ID MAGNETISM AB We consider the effect of glide-plane symmetry of the Fe-pnictogen/chalcogen layer in Fe-based superconductors on pairing in spin fluctuation models. Recent theories have proposed that so-called.-pairing states with nonzero total momentum can be realized and possess exotic properties such as odd parity spin singlet symmetry and time-reversal symmetry breaking. Here we show that. pairing is inevitable when there is orbital weight at the Fermi level from orbitals with even and odd mirror reflection symmetry in z; however, by explicit calculation, we conclude that the gap function that appears in observable quantities is identical to that found in earlier, 1 Fe per unit cell pseudocrystal momentum calculations. C1 [Wang, Y.; Berlijn, T.; Maier, T. A.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Wang, Y.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Wang, Y.; Hirschfeld, P. J.] Univ Florida, Dept Phys, Gainesville, FL 32611 USA. [Berlijn, T.; Maier, T. A.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. [Scalapino, D. J.] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA. RP Wang, Y (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RI Berlijn, Tom/A-3859-2016; Maier, Thomas/F-6759-2012 OI Berlijn, Tom/0000-0002-1001-2238; Maier, Thomas/0000-0002-1424-9996 FU Oak Ridge National Laboratory; Kavli Institute for Theoretical Physics under National Science Foundation [PHY11-25915]; [DOE DE-FG02-05ER46236,] FX The authors acknowledge their useful discussions with A. Chubukov, M. Khodas, and W. Ku. P.J.H. and Y.W. were supported by Grant No. DOE DE-FG02-05ER46236, and T.B. was supported as a Wigner Fellow at the Oak Ridge National Laboratory. A portion of this research was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. This research was supported in part by Kavli Institute for Theoretical Physics under National Science Foundation Grant No. PHY11-25915. NR 22 TC 9 Z9 9 U1 2 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 10 PY 2015 VL 114 IS 10 AR 107002 DI 10.1103/PhysRevLett.114.107002 PG 5 WC Physics, Multidisciplinary SC Physics GA CE8EE UT WOS:000352073400021 PM 25815960 ER PT J AU Bruns, DE Burtis, CA Gronowski, AM McQueen, MJ Newman, A Jonsson, JJ AF Bruns, David E. Burtis, Carl A. Gronowski, Ann M. McQueen, Matthew J. Newman, Anthony Jonsson, Jon J. CA IFCC Task Force Ethics TI Variability of ethics education in laboratory medicine training programs: Results of an international survey SO CLINICA CHIMICA ACTA LA English DT Article DE Ethics; Education; Training; Survey; Postdoctoral ID ISSUES; PATHOLOGY AB Background: Ethical considerations are increasingly important in medicine. We aimed to determine the mode and extent of teaching of ethics in training programs in clinical chemistry and laboratory medicine. Methods: We developed an on-line survey of teaching in areas of ethics relevant to laboratory medicine. Reponses were invited from directors of training programs who were recruited via email to leaders of national organizations. Results: The survey was completed by 80 directors from 24 countries who directed 113 programs. The largest numbers of respondents directed postdoctoral training of scientists (42%) or physicians (33%), post-masters degree programs (33%), and PhD programs (29%). Most programs (82%) were 2 years or longer in duration. Formal training was offered in research ethics by 39%, medical ethics by 31%, professional ethics by 24% and business ethics by 9%. The number of reported hours of formal training varied widely, e.g., from 0 to >15 h/year for research ethics and from 0 to >15 h for medical ethics. Ethics training was required and/or tested in 75% of programs that offered training. A majority (54%) of respondents reported plans to add or enhance training in ethics; many indicated a desire for online resources related to ethics, especially resources with self-assessment tools. Conclusion: Formal teaching of ethics is absent from many training programs in clinical chemistry and laboratory medicine, with heterogeneity in the extent and methods of ethics training among the programs that provide the training. A perceived need exists for online training tools, especially tools with self-assessment components. (C) 2014 The Authors. Published by Elsevier B.V. This is an open access article under the CC BY license (http://creativecommons.org/licenses/by/4.0/). C1 [Bruns, David E.] Univ Virginia, Sch Med, Dept Pathol, Charlottesville, VA 22908 USA. [Burtis, Carl A.] Oak Ridge Natl Lab, Oak Ridge, TN USA. [Gronowski, Ann M.] Washington Univ, Sch Med, Dept Pathol & Immunol, St Louis, MO USA. [McQueen, Matthew J.] McMaster Univ, Hamilton, ON L8S 4L8, Canada. [McQueen, Matthew J.] Hamilton Gen Hosp, Clin Res & Clin Trials Lab, Hamilton, ON, Canada. [Newman, Anthony] Elsevier BV, NL-1043 NX Amsterdam, Netherlands. [Jonsson, Jon J.] Univ Iceland, Fac Med, Dept Biochem & Mol Biol, Reykjavik, Iceland. [Jonsson, Jon J.] Natl Univ Hosp Iceland, Landspitali, Dept Genet & Mol Med, Reykjavik, Iceland. RP Jonsson, JJ (reprint author), Univ Iceland, Fac Med, Dept Biochem & Mol Biol, Reykjavik, Iceland. EM jonjj@hi.is NR 13 TC 1 Z9 1 U1 1 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-8981 EI 1873-3492 J9 CLIN CHIM ACTA JI Clin. Chim. Acta PD MAR 10 PY 2015 VL 442 BP 115 EP 118 DI 10.1016/j.cca.2014.11.023 PG 4 WC Medical Laboratory Technology SC Medical Laboratory Technology GA CE7TY UT WOS:000352045900022 PM 25437910 ER PT J AU Adare, A Afanasiev, S Aidala, C Ajitanand, NN Akiba, Y Akimoto, R Al-Bataineh, H Al-Ta'ani, H Alexander, J Alfred, M Andrews, KR Angerami, A Aoki, K Apadula, N Aphecetche, L Appelt, E Aramaki, Y Armendariz, R Asai, J Asano, H Aschenauer, EC Atomssa, ET Averbeck, R Awes, TC Azmoun, B Babintsev, V Bai, M Baksay, G Baksay, L Baldisseri, A Bandara, NS Bannier, B Barish, KN Barnes, PD Bassalleck, B Basye, AT Bathe, S Batsouli, S Baublis, V Baumann, C Bazilevsky, A Beaumier, M Beckman, S Belikov, S Belmont, R Ben-Benjamin, J Bennett, R Berdnikov, A Berdnikov, Y Bhom, JH Bickley, AA Black, D Blau, DS Boissevain, JG Bok, JS Borel, H Boyle, K Brooks, ML Broxmeyer, D Bryslawskyj, J Buesching, H Bumazhnov, V Bunce, G Butsyk, S Camacho, CM Campbell, S Caringi, A Castera, P Chang, BS Chang, WC Charvet, JL Chen, CH Chernichenko, S Chi, CY Chiu, M Choi, IJ Choi, JB Choudhury, RK Christiansen, P Chujo, T Chung, P Churyn, A Chvala, O Cianciolo, V Citron, Z Cole, BA del Valle, ZC Connors, M Constantin, P Csanad, M Csorgo, T Dahms, T Dairaku, S Danchev, I Das, K Datta, A Daugherity, MS David, G Dayananda, MK DeBlasio, K Dehmelt, K Denisov, A d'Enterria, D Deshpande, A Desmond, EJ Dharmawardane, KV Dietzsch, O Ding, L Dion, A Do, JH Donadelli, M Drapier, O Drees, A Drees, KA Dubey, AK Durham, JM Durum, A Dutta, D Dzhordzhadze, V D'Orazio, L Edwards, S Efremenko, YV Ellinghaus, F Engelmore, T Enokizono, A En'yo, H Esumi, S Eyser, KO Fadem, B Feege, N Fields, DE Finger, M Finger, M Fleuret, F Fokin, SL Fraenkel, Z Frantz, JE Franz, A Frawley, AD Fujiwara, K Fukao, Y Fusayasu, T Gal, C Gallus, P Garg, P Garishvili, I Ge, H Giordano, F Glenn, A Gong, H Gong, X Gonin, M Gosset, J Goto, Y de Cassagnac, RG Grau, N Greene, SV Grim, G Perdekamp, MG Gu, Y Gunji, T Guo, L Guragain, H Gustafsson, HA Hachiya, T Henni, AH Haggerty, JS Hahn, KI Hamagaki, H Hamblen, J Han, R Han, SY Hanks, J Harper, C Hartouni, EP Haruna, K Hasegawa, S Hashimoto, K Haslum, E Hayano, R He, X Heffner, M Hemmick, TK Hester, T Hill, JC Hohlmann, M Hollis, RS Holzmann, W Homma, K Hong, B Horaguchi, T Hori, Y Hornback, D Hoshino, T Huang, J Huang, S Ichihara, T Ichimiya, R Iinuma, H Ikeda, Y Imai, K Imazu, Y Imrek, J Inaba, M Iordanova, A Isenhower, D Ishihara, M Isobe, T Issah, M Isupov, A Ivanischev, D Ivanishchev, D Iwanaga, Y Jacak, BV Jeon, SJ Jezghani, M Jia, J Jiang, X Jin, J John, D Johnson, BM Jones, T Joo, E Joo, KS Jouan, D Jumper, DS Kajihara, F Kametani, S Kamihara, N Kamin, J Kaneti, S Kang, BH Kang, JH Kang, JS Kapustinsky, J Karatsu, K Kasai, M Kawall, D Kawashima, M Kazantsev, AV Kempel, T Key, JA Khachatryan, V Khanzadeev, A Kihara, K Kijima, KM Kikuchi, J Kim, A Kim, BI Kim, C Kim, DH Kim, DJ Kim, E Kim, EJ Kim, HJ Kim, M Kim, SH Kim, YJ Kim, YK Kinney, E Kiriluk, K Kiss, A Kistenev, E Klatsky, J Klay, J Klein-Boesing, C Kleinjan, D Kline, P Koblesky, T Kochenda, L Kofarago, M Komkov, B Konno, M Koster, J Kotov, D Kozlov, A Kral, A Kravitz, A Kunde, GJ Kurita, K Kurosawa, M Kweon, MJ Kwon, Y Kyle, GS Lacey, R Lai, YS Lajoie, JG Layton, D Lebedev, A Lee, DM Lee, J Lee, KB Lee, KS Lee, SH Lee, SR Lee, T Leitch, MJ Leite, MAL Leitgab, M Lenzi, B Li, X Lichtenwalner, P Liebing, P Lim, SH Levy, LAL Liska, T Litvinenko, A Liu, H Liu, MX Love, B Lynch, D Maguire, CF Makdisi, YI Makek, M Malakhov, A Malik, MD Manion, A Manko, VI Mannel, E Mao, Y Masek, L Masui, H Matathias, F McCumber, M McGaughey, PL McGlinchey, D McKinney, C Means, N Meles, A Mendoza, M Meredith, B Miake, Y Mibe, T Mignerey, AC Mikes, P Miki, K Miller, AJ Milov, A Mishra, DK Mishra, M Mitchell, JT Miyachi, Y Miyasaka, S Mizuno, S Mohanty, AK Montuenga, P Moon, HJ Moon, T Morino, Y Morreale, A Morrison, DP Motschwiller, S Moukhanova, TV Mukhopadhyay, D Murakami, T Murata, J Mwai, A Nagamiya, S Nagle, JL 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Savastio, M Sawada, S Schaefer, B Schmoll, BK Sedgwick, K Seele, J Seidl, R Semenov, AY Semenov, V Sen, A Seto, R Sett, P Sexton, A Sharma, D Shein, I Shibata, TA Shigaki, K Shim, HH Shimomura, M Shoji, K Shukla, P Sickles, A Silva, CL Silvermyr, D Silvestre, C Sim, KS Singh, BK Singh, CP Singh, V Slunecka, M Sodre, T Soldatov, A Soltz, RA Sondheim, WE Sorensen, SP Sourikova, IV Staley, F Stankus, PW Stenlund, E Stepanov, M Ster, A Stoll, SP Sugitate, T Suire, C Sukhanov, A Sumita, T Sun, J Sziklai, J Takagui, EM Takahara, A Taketani, A Tanabe, R Tanaka, Y Taneja, S Tanida, K Tannenbaum, MJ Tarafdar, S Taranenko, A Tarjan, P Tennant, E Themann, H Thomas, D Thomas, TL Timilsina, A Todoroki, T Togawa, M Toia, A Tomasek, L Tomasek, M Tomita, Y Torii, H Towell, M Towell, R Towell, RS Tram, VN Tserruya, I Tsuchimoto, Y Utsunomiya, K Vale, C Valle, H van Hecke, HW Vargyas, M Vazquez-Zambrano, E Veicht, A Velkovska, J Vertesi, R Vinogradov, AA Virius, M Vossen, A Vrba, V Vznuzdaev, E Wang, XR Watanabe, D Watanabe, K Watanabe, Y Watanabe, YS Wei, F Wei, R Wessels, J Whitaker, S White, SN Winter, D Wolin, S Woody, CL Wright, RM Wysocki, M Xia, B Xie, W Xue, L Yalcin, S Yamaguchi, YL Yamaura, K Yang, R Yanovich, A Ying, J Yokkaichi, S Yoo, JS Yoon, I You, Z Young, GR Younus, I Yushmanov, IE Zajc, WA Zaudtke, O Zelenski, A Zhang, C Zhou, S Zolin, L AF Adare, A. Afanasiev, S. Aidala, C. Ajitanand, N. N. Akiba, Y. Akimoto, R. Al-Bataineh, H. Al-Ta'ani, H. Alexander, J. Alfred, M. Andrews, K. R. Angerami, A. Aoki, K. Apadula, N. Aphecetche, L. Appelt, E. Aramaki, Y. Armendariz, R. Asai, J. Asano, H. Aschenauer, E. C. Atomssa, E. T. Averbeck, R. Awes, T. C. Azmoun, B. Babintsev, V. Bai, M. Baksay, G. Baksay, L. Baldisseri, A. Bandara, N. S. Bannier, B. Barish, K. N. Barnes, P. D. Bassalleck, B. Basye, A. T. Bathe, S. Batsouli, S. Baublis, V. Baumann, C. Bazilevsky, A. Beaumier, M. Beckman, S. Belikov, S. Belmont, R. Ben-Benjamin, J. Bennett, R. Berdnikov, A. Berdnikov, Y. Bhom, J. H. Bickley, A. A. Black, D. Blau, D. S. Boissevain, J. G. Bok, J. S. Borel, H. Boyle, K. Brooks, M. L. Broxmeyer, D. Bryslawskyj, J. Buesching, H. Bumazhnov, V. Bunce, G. Butsyk, S. Camacho, C. M. Campbell, S. Caringi, A. Castera, P. Chang, B. S. Chang, W. C. Charvet, J. -L. Chen, C. -H. Chernichenko, S. Chi, C. Y. Chiu, M. Choi, I. J. Choi, J. B. Choudhury, R. K. 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Sourikova, I. V. Staley, F. Stankus, P. W. Stenlund, E. Stepanov, M. Ster, A. Stoll, S. P. Sugitate, T. Suire, C. Sukhanov, A. Sumita, T. Sun, J. Sziklai, J. Takagui, E. M. Takahara, A. Taketani, A. Tanabe, R. Tanaka, Y. Taneja, S. Tanida, K. Tannenbaum, M. J. Tarafdar, S. Taranenko, A. Tarjan, P. Tennant, E. Themann, H. Thomas, D. Thomas, T. L. Timilsina, A. Todoroki, T. Togawa, M. Toia, A. Tomasek, L. Tomasek, M. Tomita, Y. Torii, H. Towell, M. Towell, R. Towell, R. S. Tram, V-N. Tserruya, I. Tsuchimoto, Y. Utsunomiya, K. Vale, C. Valle, H. van Hecke, H. W. Vargyas, M. Vazquez-Zambrano, E. Veicht, A. Velkovska, J. Vertesi, R. Vinogradov, A. A. Virius, M. Vossen, A. Vrba, V. Vznuzdaev, E. Wang, X. R. Watanabe, D. Watanabe, K. Watanabe, Y. Watanabe, Y. S. Wei, F. Wei, R. Wessels, J. Whitaker, S. White, S. N. Winter, D. Wolin, S. Woody, C. L. Wright, R. M. Wysocki, M. Xia, B. Xie, W. Xue, L. Yalcin, S. Yamaguchi, Y. L. Yamaura, K. Yang, R. Yanovich, A. Ying, J. Yokkaichi, S. Yoo, J. S. Yoon, I. You, Z. Young, G. R. Younus, I. Yushmanov, I. E. Zajc, W. A. Zaudtke, O. Zelenski, A. Zhang, C. Zhou, S. Zolin, L. CA PHENIX Collaboration TI Search for dark photons from neutral meson decays in p plus p and d plus Au collisions at root s(NN)=200 GeV SO PHYSICAL REVIEW C LA English DT Article ID DETECTOR; ENERGIES; PROTON; RAYS AB The standard model (SM) of particle physics is spectacularly successful, yet the measured value of the muon anomalous magnetic moment (g - 2)mu deviates from SM calculations by 3.6 sigma. Several theoretical models attribute this to the existence of a "dark photon," an additional U(1) gauge boson, which is weakly coupled to ordinary photons. The PHENIX experiment at the Relativistic Heavy Ion Collider has searched for a dark photon, U, in pi(0), eta -> gamma e(+)e(-) decays and obtained upper limits of O(2 x 10(-6)) on U-gamma mixing at 90% C.L. for the mass range 30 < m(U) < 90 MeV/c(2). Combined with other experimental limits, the remaining region in the U-gamma mixing parameter space that can explain the (g - 2)(mu) deviation from its SM value is nearly completely excluded at the 90% confidence level, with only a small region of 29 < m(U) < 32 MeV/c(2) remaining. C1 [Andrews, K. R.; Basye, A. T.; Daugherity, M. S.; Isenhower, D.; Jones, T.; Jumper, D. S.; Miller, A. J.; Pinson, R.; Thomas, D.; Towell, M.; Towell, R.; Towell, R. S.; Wright, R. M.] Abilene Christian Univ, Abilene, TX 79699 USA. [Chang, W. C.] Acad Sinica, Inst Phys, Taipei 11529, Taiwan. [Grau, N.] Augustana Coll, Dept Phys, Sioux Falls, SD 57197 USA. [Garg, P.; Mishra, M.; Singh, B. K.; Singh, C. P.; Singh, V.; Tarafdar, S.] Banaras Hindu Univ, Dept Phys, Varanasi 221005, Uttar Pradesh, India. [Choudhury, R. K.; Dutta, D.; Mishra, D. K.; Mohanty, A. K.; Netrakanti, P. K.; Sett, P.; Shukla, P.] Bhabha Atom Res Ctr, Bombay 400085, Maharashtra, India. [Bathe, S.; Bryslawskyj, J.; Rowan, Z.] CUNY, Baruch Coll, New York, NY 10010 USA. [Bai, M.; Drees, K. A.; Makdisi, Y. I.; Zelenski, A.] Brookhaven Natl Lab, Collider Accelerator Dept, Upton, NY 11973 USA. [Aschenauer, E. C.; Azmoun, B.; Bazilevsky, A.; Belikov, S.; Buesching, H.; Bunce, G.; Chiu, M.; David, G.; Desmond, E. J.; Franz, A.; Haggerty, J. S.; Huang, J.; Jia, J.; Johnson, B. M.; Kistenev, E.; Lynch, D.; Mannel, E.; Milov, A.; Mitchell, J. T.; Morrison, D. P.; Nouicer, R.; O'Brien, E.; Pak, R.; Perepelitsa, D. V.; Petti, R.; Pinkenburg, C.; Pisani, R. P.; Purschke, M. L.; Sakaguchi, T.; Sickles, A.; Sourikova, I. V.; Stoll, S. P.; Sukhanov, A.; Tannenbaum, M. J.; Vale, C.; White, S. N.; Woody, C. L.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Armendariz, R.; Barish, K. N.; Bathe, S.; Beaumier, M.; Black, D.; Chvala, O.; Dzhordzhadze, V.; Eyser, K. O.; Hester, T.; Hollis, R. S.; Iordanova, A.; Kleinjan, D.; Mendoza, M.; Morreale, A.; Rolnick, S. 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RP Adare, A (reprint author), Abilene Christian Univ, Abilene, TX 79699 USA. EM morrison@bnl.gov; jamie.nagle@colorado.edu RI Hayano, Ryugo/F-7889-2012; HAMAGAKI, HIDEKI/G-4899-2014; Gu, Yi/B-6101-2016; Durum, Artur/C-3027-2014; Sen, Abhisek/J-1157-2016; Nattrass, Christine/J-6752-2016; Sorensen, Soren /K-1195-2016; Yokkaichi, Satoshi/C-6215-2017; Taketani, Atsushi/E-1803-2017; Semenov, Vitaliy/E-9584-2017 OI Hayano, Ryugo/0000-0002-1214-7806; Gu, Yi/0000-0003-4467-697X; Sen, Abhisek/0000-0003-1192-3938; Nattrass, Christine/0000-0002-8768-6468; Sorensen, Soren /0000-0002-5595-5643; Taketani, Atsushi/0000-0002-4776-2315; FU Office of Nuclear Physics in the Office of Science of the Department of Energy; National Science Foundation; Renaissance Technologies LLC; Abilene Christian University Research Council; Research Foundation of SUNY; Ministry of Education, Culture, Sports, Science, and Technology; Japan Society for the Promotion of Science (Japan); Conselho Nacional de Desenvolvimento Cientifico e Tecnologico; Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (Brazil); Natural Science Foundation of China (People's Republic of China); Ministry of Science, Education, and Sports (Croatia); Ministry of Education, Youth and Sports (Czech Republic); Centre National de la Recherche Scientifique (France); Commissariat a l'Energie Atomique (France); Institut National de Physique Nucleaire et de Physique des Particules (France); Bundesministerium fur Bildung und Forschung (Germany); Deutscher Akademischer Austausch Dienst (Germany); Alexander von Humboldt Stiftung (Germany); OTKA [NK 101 428]; Ch. Simonyi Fund (Hungary); Department of Atomic Energy (India); Department of Science and Technology (India); Israel Science Foundation (Israel); NRF of the Ministry of Education (Korea); Physics Department, Lahore University of Management Sciences (Pakistan); Ministry of Education and Science (Russia); Russian Academy of Sciences (Russia); Federal Agency of Atomic Energy (Russia); VR (Sweden); Wallenberg Foundation (Sweden); U.S. Civilian Research and Development Foundation for the Independent States of the Former Soviet Union; Hungarian American Enterprise Scholarship Fund; U.S.-Israel Binational Science Foundation FX We thank the staff of the Collider-Accelerator and Physics Departments at Brookhaven National Laboratory and the staff of the other PHENIX participating institutions for their vital contributions. We also thank William Marciano and Hye-Sung Lee for useful discussions and theoretical calculations, and we thank the WASA, HADES, and BABAR collaborations for useful interactions. We acknowledge support from the Office of Nuclear Physics in the Office of Science of the Department of Energy, the National Science Foundation, a sponsored research grant from Renaissance Technologies LLC, Abilene Christian University Research Council, Research Foundation of SUNY, and Dean of the College of Arts and Sciences, Vanderbilt University (U.S.A.); Ministry of Education, Culture, Sports, Science, and Technology and the Japan Society for the Promotion of Science (Japan); Conselho Nacional de Desenvolvimento Cientifico e Tecnologico and Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (Brazil); Natural Science Foundation of China (People's Republic of China); Ministry of Science, Education, and Sports (Croatia); Ministry of Education, Youth and Sports (Czech Republic); Centre National de la Recherche Scientifique, Commissariat a l'Energie Atomique, and Institut National de Physique Nucleaire et de Physique des Particules (France); Bundesministerium fur Bildung und Forschung, Deutscher Akademischer Austausch Dienst, and Alexander von Humboldt Stiftung (Germany); OTKA Grant No. NK 101 428 and the Ch. Simonyi Fund (Hungary); Department of Atomic Energy and Department of Science and Technology (India); Israel Science Foundation (Israel); Basic Science Research Program through NRF of the Ministry of Education (Korea); Physics Department, Lahore University of Management Sciences (Pakistan); Ministry of Education and Science, Russian Academy of Sciences, Federal Agency of Atomic Energy (Russia); VR and Wallenberg Foundation (Sweden); the U.S. Civilian Research and Development Foundation for the Independent States of the Former Soviet Union; the Hungarian American Enterprise Scholarship Fund; and the U.S.-Israel Binational Science Foundation. NR 35 TC 17 Z9 18 U1 7 U2 35 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD MAR 10 PY 2015 VL 91 IS 3 AR 031901 DI 10.1103/PhysRevC.91.031901 PG 8 WC Physics, Nuclear SC Physics GA CE7LN UT WOS:000352021800001 ER PT J AU Chang, C Busha, MT Wechsler, RH Refregier, A Amara, A Rykoff, E Becker, MR Bruderer, C Gamper, L Leistedt, B Peiris, H Abbott, T Abdalla, FB Balbinot, E Banerji, M Bernstein, RA Bertin, E Brooks, D Carner, A Desai, S da Costa, LN Cunha, CE Eifler, T Evrard, AE Neto, AR Gerdes, D Gruen, D James, D Kuehn, K Maia, MAG Makler, M Ogando, R Plazas, A Sanchez, E Santiago, B Schubnell, M Sevilla-Noarbe, I Smith, C Soares-Santos, M Suchyta, E Swanson, MEC Tarle, G Zuntz, J AF Chang, C. Busha, M. T. Wechsler, R. H. Refregier, A. Amara, A. Rykoff, E. Becker, M. R. Bruderer, C. Gamper, L. Leistedt, B. Peiris, H. Abbott, T. Abdalla, F. B. Balbinot, E. Banerji, M. Bernstein, R. A. Bertin, E. Brooks, D. Carner, A. Desai, S. da Costa, L. N. Cunha, C. E. Eifler, T. Evrard, A. E. Rausti Neto, A. Gerdes, D. Gruen, D. James, D. Kuehn, K. Maia, M. A. G. Makler, M. Ogando, R. Plazas, A. Sanchez, E. Santiago, B. Schubnell, M. Sevilla-Noarbe, I. Smith, C. Soares-Santos, M. Suchyta, E. Swanson, M. E. C. Tarle, G. Zuntz, J. TI MODELING THE TRANSFER FUNCTION FOR THE DARK ENERGY SURVEY SO ASTROPHYSICAL JOURNAL LA English DT Article DE methods: data analysis; methods: numerical; surveys; techniques: image processing ID RESOLVED STELLAR POPULATIONS; STAR-GALAXY CLASSIFICATION; IMAGE-ANALYSIS; COSMIC SHEAR; MONTE-CARLO; WIDE-FIELD; SIMULATIONS; CATALOG; CLUSTERS; SYSTEMATICS AB We present a forward-modeling simulation framework designed to model the data products from the Dark Energy Survey (DES). This forward-model process can be thought of as a transfer function-amapping from cosmological/astronomical signals to the final data products used by the scientists. Using output from the cosmological simulations (the Blind Cosmology Challenge), we generate simulated images (the Ultra Fast Image Simulator) and catalogs representative of the DES data. In this work we demonstrate the framework by simulating the 244 deg(2) coadd images and catalogs in five bands for the DES Science Verification data. The simulation output is compared with the corresponding data to show that major characteristics of the images and catalogs can be captured. We also point out several directions of future improvements. Two practical examples-star-galaxy classification and proximity effects on object detection-are then used to illustrate how one can use the simulations to address systematics issues in data analysis. With clear understanding of the simplifications in our model, we show that one can use the simulations side-by-side with data products to interpret the measurements. This forward modeling approach is generally applicable for other upcoming and future surveys. It provides a powerful tool for systematics studies that is sufficiently realistic and highly controllable. C1 [Chang, C.; Refregier, A.; Amara, A.; Bruderer, C.; Gamper, L.] ETH, Dept Phys, CH-8093 Zurich, Switzerland. [Busha, M. T.; Wechsler, R. H.; Rykoff, E.; Becker, M. R.] Kavli Inst Particle Astrophys & Cosmol, Stanford, CA 94305 USA. [Busha, M. T.; Wechsler, R. H.; Rykoff, E.; Becker, M. R.] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Wechsler, R. H.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Leistedt, B.; Peiris, H.; Abdalla, F. B.; Brooks, D.] UCL, Dept Phys & Astron, London WC1E 6BT, England. [Abbott, T.; James, D.; Smith, C.] Natl Opt Astron Observ, Cerro Tololo Inter Amer Observ, La Serena, Chile. [Abdalla, F. B.] Rhodes Univ, Dept Phys & Elect, ZA-6140 Grahamstown, South Africa. [Balbinot, E.] Univ Surrey, Dept Phys, Guildford GU2 7XH, Surrey, England. [Banerji, M.] Univ Cambridge, Inst Astron, Cambridge CB3 0HA, England. [Banerji, M.] Univ Cambridge, Kavli Inst Cosmol, Cambridge CB3 0HA, England. [Bernstein, R. A.] Carnegie Observa, Pasadena, CA 91101 USA. [Bertin, E.; Evrard, A. E.] Univ Paris 06, Inst Astrophys Paris, F-75014 Paris, France. [Bertin, E.; Evrard, A. E.] CNRS, UMR7095, F-75014 Paris, France. [Carner, A.; da Costa, L. N.; Maia, M. A. G.; Ogando, R.] Observ Nacl, BR-20921400 Rio De Janeiro, RJ, Brazil. [Carner, A.; da Costa, L. N.; Rausti Neto, A.; Maia, M. A. G.; Ogando, R.; Santiago, B.] Lab Interinstituc & Astron LIneA, BR-20921400 Rio De Janeiro, RJ, Brazil. [Desai, S.] Univ Munich, Dept Phys, D-81679 Munich, Germany. [Desai, S.] Excellence Cluster Universe, D-85748 Garching, Germany. [Cunha, C. E.] Robert Bosch LLC, Palo Alto, CA 94304 USA. [Eifler, T.] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Evrard, A. E.; Gerdes, D.; Schubnell, M.; Tarle, G.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Evrard, A. E.] Univ Michigan, Dept Astron, Ann Arbor, MI 48109 USA. [Gruen, D.] Univ Observ Munich, D-81679 Munich, Germany. [Gruen, D.] Max Planck Inst Extraterr Phys, D-85748 Garching, Germany. [Kuehn, K.] Australian Astron Observ, N Ryde, NSW 2113, Australia. [Makler, M.] ICRA, Ctr Brasileiro Pesquisas Fis, BR-22290180 Rio De Janeiro, RJ, Brazil. [Plazas, A.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Sanchez, E.; Sevilla-Noarbe, I.] CIEMAT, Madrid, Spain. [Santiago, B.] Univ Fed Rio Grande do Sul, Inst Fis, BR-91501970 Porto Alegre, RS, Brazil. [Soares-Santos, M.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Suchyta, E.] Ohio State Univ, Ctr Cosmol & Astro Particle Phys, Columbus, OH 43210 USA. [Swanson, M. E. C.] Natl Ctr Supercomp Applicat, Urbana, IL 61801 USA. [Zuntz, J.] Univ Manchester, Sch Phys & Astron, Jodrell Bank Ctr Astrophys, Manchester M13 9PL, Lancs, England. RP Chang, C (reprint author), ETH, Dept Phys, Wolfgang Pauli Str 16, CH-8093 Zurich, Switzerland. RI Balbinot, Eduardo/E-8019-2015; Ogando, Ricardo/A-1747-2010; da Costa, Luiz Alberto/I-1326-2013; Makler, Martin/G-2639-2012; Sanchez, Eusebio/H-5228-2015; OI Becker, Matthew/0000-0001-7774-2246; Suchyta, Eric/0000-0002-7047-9358; Balbinot, Eduardo/0000-0002-1322-3153; Ogando, Ricardo/0000-0003-2120-1154; Evrard, August/0000-0002-4876-956X; Chang, Chihway/0000-0002-7887-0896; Banerji, Manda/0000-0002-0639-5141; da Costa, Luiz Alberto/0000-0002-7731-277X; Makler, Martin/0000-0003-2206-2651; Sanchez, Eusebio/0000-0002-9646-8198; Abdalla, Filipe/0000-0003-2063-4345 FU Swiss National Science Foundation [200021-149442, 200021-143906]; Department of Energy contract [DE-AC3-76SF00515]; Perren Fund; IMPACT Fund; STFC; European Research Council under the European Community's Seventh Framework Programme (FP7)/ERC [306478]; PROGRAMA DE APOIO AO POS-DOUTORADO NO ESTADO DO RIO DE JANEIRO - PAPDRJ; SFB-Transregio 33 "The Dark Universe" by the Deutsche Forschungsgemeinschaft (DFG); DFG cluster of excellence "Origin and Structure of the Universe"; DOE [DE-AC02-98CH10886]; European Research Council in the form of a Starting Grant [240672]; U.S. Department of Energy; U.S. National Science Foundation; Ministry of Science and Education of Spain; Science and Technology Facilities Council of the United Kingdom; Higher Education Funding Council for England; National Center for Supercomputing Applications at the University of Illinois at Urbana-Champaign; Kavli Institute of Cosmological Physics at the University of Chicago; Financiadora de Estudos e Projetos; Fundacao Carlos Chagas Filho de Amparo a Pesquisa do Estado do Rio de Janeiro; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico and the Ministerio da Ciencia e Tecnologia; Deutsche Forschungsgemeinschaft; Collaborating Institutions in the Dark Energy Survey FX We thank Gary Bernstein, Eric Huff, Tesla Jeltema, Huan Lin, and Felipe Menanteau for helpful comments and discussions on the paper. C.C., A.R., A. A., and C.B. are supported by the Swiss National Science Foundation grants 200021-149442 and 200021-143906. M.T.B., R.H.W., E.R., and M.R.B. acknowledge support from the Department of Energy contract to SLAC National Accelerator Laboratory No. DE-AC3-76SF00515. B.L. is supported by the Perren Fund and the IMPACT Fund. H.V.P. is supported by STFC and the European Research Council under the European Community's Seventh Framework Programme (FP7/2007-2013)/ERC grant agreement No. 306478-CosmicDawn. A.C.R. is supported by the PROGRAMA DE APOIO AO POS-DOUTORADO NO ESTADO DO RIO DE JANEIRO - PAPDRJ. D.G. was supported by SFB-Transregio 33 "The Dark Universe" by the Deutsche Forschungsgemeinschaft (DFG) and the DFG cluster of excellence "Origin and Structure of the Universe." A.P. is supported by DOE grant DE-AC02-98CH10886. J.Z. acknowledges support from the European Research Council in the form of a Starting Grant with number 240672.; Funding for the DES Projects has been provided by the U.S. Department of Energy, the U.S. National Science Foundation, the Ministry of Science and Education of Spain, the Science and Technology Facilities Council of the United Kingdom, the Higher Education Funding Council for England, the National Center for Supercomputing Applications at the University of Illinois at Urbana-Champaign, the Kavli Institute of Cosmological Physics at the University of Chicago, Financiadora de Estudos e Projetos, Fundacao Carlos Chagas Filho de Amparo a Pesquisa do Estado do Rio de Janeiro, Conselho Nacional de Desenvolvimento Cientifico e Tecnologico and the Ministerio da Ciencia e Tecnologia, the Deutsche Forschungsgemeinschaft and the Collaborating Institutions in the Dark Energy Survey. NR 72 TC 13 Z9 13 U1 1 U2 6 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAR 10 PY 2015 VL 801 IS 2 AR 73 DI 10.1088/0004-637X/801/2/73 PG 14 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CD3GE UT WOS:000350965500002 ER PT J AU Gray, WJ Scannapieco, E Kasen, D AF Gray, William J. Scannapieco, Evan Kasen, Daniel TI ATOMIC CHEMISTRY IN TURBULENT ASTROPHYSICAL MEDIA. I. EFFECT OF ATOMIC COOLING SO ASTROPHYSICAL JOURNAL LA English DT Article DE astrochemistry; ISM: abundances; ISM: atoms; turbulence ID FINITE-DENSITY PLASMAS; DIELECTRONIC RECOMBINATION DATA; COS-HALOS SURVEY; PROBABILITY-DISTRIBUTION FUNCTIONS; REDSHIFT CIRCUMGALACTIC MEDIUM; DIRECT NUMERICAL-SIMULATION; MACH NUMBER RELATION; ISOELECTRONIC SEQUENCE; INTERSTELLAR-MEDIUM; STAR-FORMATION AB We carry out direct numerical simulations of turbulent astrophysical media that explicitly track ionizations, recombinations, and species-by-species radiative cooling. The simulations assume solar composition and follows the evolution of hydrogen, helium, carbon, oxygen, sodium, and magnesium, but they do not include the presence of an ionizing background. In this case, the medium reaches a global steady state that is purely a function of the one-dimensional turbulent velocity dispersion, sigma(1D), and the product of the mean density and the driving scale of turbulence, nL. Our simulations span a grid of models with s1D ranging from 6 to 58 km s(-1) and nL ranging from 1016 to 1020 cm(-2), which correspond to turbulent Mach numbers from M - 0.2 to 10.6. The species abundances are well described by single-temperature estimates whenever M is small, but local equilibrium models can not accurately predict the global equilibrium abundances when M greater than or similar to 1. To allow future studies to account for nonequilibrium effects in turbulent media, we gather our results into a series of tables, which we will extend in the future to encompass a wider range of elements, compositions, and ionizing processes. C1 [Gray, William J.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Scannapieco, Evan] Arizona State Univ, Sch Earth & Space Explorat, Tempe, AZ 85287 USA. [Kasen, Daniel] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Kasen, Daniel] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. RP Gray, WJ (reprint author), Lawrence Livermore Natl Lab, POB 808,L-038, Livermore, CA 94550 USA. FU NSF [AST11-03608, PHY11-25915]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX We would like to thank Christopher Matzner, Cody Raskin, Eve Ostriker, Robert J. Thacker, and David Williamson for helpful discussions. ES gratefully acknowledges Joanne Cohn, Eliott Quatert, and the UC Berkeley Theoretical Astronomy Center, Uros Seljak and the Lawrence Berkeley National Lab Cosmology group, and the organizers of the Gravitys Loyal Opposition: The Physics of Star Formation Feedback at the Kavli Institute for Theoretical Physics, for hosting him during the period when much of this work was carried out. The software used in this work was in part developed by the DOE NNSA-ASC OASCR Flash Center at the University of Chicago. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. LLNL-JRNL-662155. ES was supported by NSF grant AST11-03608, and PHY11-25915. The figures and analysis presented here were created using the yt analysis package (Turk et al. 2011). NR 71 TC 4 Z9 4 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAR 10 PY 2015 VL 801 IS 2 AR 107 DI 10.1088/0004-637X/801/2/107 PG 16 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CD3GE UT WOS:000350965500036 ER PT J AU Xu, Y Newberg, HJ Carlin, JL Liu, C Deng, LC Li, J Schonrich, R Yanny, B AF Xu, Yan Newberg, Heidi Jo Carlin, Jeffrey L. Liu, Chao Deng, Licai Li, Jing Schoenrich, Ralph Yanny, Brian TI RINGS AND RADIAL WAVES IN THE DISK OF THE MILKY WAY SO ASTROPHYSICAL JOURNAL LA English DT Article DE Galaxy: disk; Galaxy: kinematics and dynamics; Galaxy: structure ID DIGITAL SKY SURVEY; EXPLORING HALO SUBSTRUCTURE; TRIANGULUM-ANDROMEDA REGION; GALACTIC DISK; DATA RELEASE; GIANT STARS; CANIS-MAJOR; VERTICAL-DISTRIBUTION; STELLAR STRUCTURES; GALAXY FORMATION AB We show that in the anticenter region, between Galactic longitudes of 110 degrees < l < 229 degrees, there is an oscillating asymmetry in the main-sequence star counts on either side of the Galactic plane using data from the Sloan Digital Sky Survey. This asymmetry oscillates from more stars in the north at distances of about 2 kpc from the Sun to more stars in the south at 4-6 kpc from the Sun to more stars in the north at distances of 8-10 kpc from the Sun. We also see evidence that there are more stars in the south at distances of 12-16 kpc from the Sun. The three more distant asymmetries form roughly concentric rings around the Galactic center, opening in the direction of the Milky Way's spiral arms. The northern ring, 9 kpc from the Sun, is easily identified with the previously discovered Monoceros Ring. Parts of the southern ring at 14 kpc from the Sun (which we call the TriAnd Ring) have previously been identified as related to the Monoceros Ring, and others have been called the Triangulum Andromeda Overdensity. The two nearer oscillations are approximated by a toy model in which the disk plane is offset by the order of 100 pc up and then down at different radii. We also show that the disk is not azimuthally symmetric around the Galactic anticenter and that there could be a correspondence between our observed oscillations and the spiral structure of the Galaxy. Our observations suggest that the TriAnd and Monoceros Rings (which extend to at least 25 kpc from the Galactic center) are primarily the result of disk oscillations. C1 [Xu, Yan; Liu, Chao; Deng, Licai] Chinese Acad Sci, Natl Astron Observ, Key Lab Opt Astron, Beijing 100012, Peoples R China. [Xu, Yan; Newberg, Heidi Jo; Carlin, Jeffrey L.] Rensselaer Polytech Inst, Dept Phys Appl Phys & Astron, Troy, NY 12180 USA. [Li, Jing] Chinese Acad Sci, Shanghai Astron Observ, Shanghai 200030, Peoples R China. [Schoenrich, Ralph] Univ Oxford, Rudolf Peierls Ctr Theoret Phys, Oxford OX1 3NP, England. [Yanny, Brian] Fermilab Natl Accelerator Lab, Expt Astrophys Grp, Batavia, IL 60510 USA. RP Xu, Y (reprint author), Chinese Acad Sci, Natl Astron Observ, Key Lab Opt Astron, Datun Rd 20A, Beijing 100012, Peoples R China. EM xuyan@bao.ac.en OI Carlin, Jeffrey/0000-0002-3936-9628 FU NSFC grant [11203030]; National Key Basic Research Program of China [2014CB845703]; U.S. National Science Foundation [AST 09-37523, AST 14-09421]; Youth Innovation Promotion Association, CAS; Alfred P. Sloan Foundation; National Science Foundation; U.S. Department of Energy Office of Science; Participating Institutions FX This work is supported by NSFC grant No. 11203030 and the National Key Basic Research Program of China 2014CB845703, as well as the U.S. National Science Foundation under grants AST 09-37523 and AST 14-09421. We are thankful for funding from the Youth Innovation Promotion Association, CAS. We thank the anonymous referee for comments that led to a clearer presentation of our results. Funding for SDSS-III has been provided by the Alfred P. Sloan Foundation, the Participating Institutions, the National Science Foundation, and the U.S. Department of Energy Office of Science. The SDSS-III Web site is http://sdss3.org/. SDSS-III is managed by the Astrophysical Research Consortium for the Participating Institutions of the SDSS-III Collaboration, including the University of Arizona, the Brazilian Participation Group, Brookhaven National Laboratory, Carnegie Mellon University, University of Florida, the French Participation Group, the German Participation Group, Harvard University, the Instituto de Astrofisica de Canarias, the Michigan State/Notre Dame/JINA Participation Group, Johns Hopkins University, Lawrence Berkeley National Laboratory, Max Planck Institute for Astrophysics, Max Planck Institute for Extraterrestrial Physics, New Mexico State University, New York University, Ohio State University, Pennsylvania State University, University of Portsmouth, Princeton University, the Spanish Participation Group, University of Tokyo, University of Utah, Vanderbilt University, University of Virginia, University of Washington, and Yale University. NR 72 TC 28 Z9 28 U1 0 U2 6 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAR 10 PY 2015 VL 801 IS 2 AR 105 DI 10.1088/0004-637X/801/2/105 PG 25 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CD3GE UT WOS:000350965500034 ER PT J AU Singh, A Coughlan, C Milliron, DJ Ryan, KM AF Singh, Ajay Coughlan, Claudia Milliron, Delia J. Ryan, Kevin M. TI Solution Synthesis and Assembly of Wurtzite-Derived Cu-In-Zn-S Nanorods with Tunable Composition and Band Gap SO CHEMISTRY OF MATERIALS LA English DT Article ID CORE/SHELL QUANTUM DOTS; LIQUID-AIR INTERFACE; COLLOIDAL SYNTHESIS; SEMICONDUCTOR NANOCRYSTALS; SOLAR-CELLS; CHALCOGENIDE NANOCRYSTALS; THERMOELECTRIC PROPERTIES; CATION-EXCHANGE; SHAPE CONTROL; FILMS AB We report a low-energy colloidal synthesis route to homogeneously alloyed Cu-In-Zn-S nanorods that have the wurtzite crystal structure and demonstrate that the optical band gap of these nanorods is compositionally tunable through direct control of the zinc precursor molar ratio. The as-synthesized nanorods are highly monodisperse and can be assembled in both lateral and perpendicular arrays at the liquid-air interface. C1 [Singh, Ajay; Coughlan, Claudia; Ryan, Kevin M.] Univ Limerick, MSSI, Limerick, Ireland. [Singh, Ajay; Coughlan, Claudia; Ryan, Kevin M.] Univ Limerick, Dept Chem & Environm Sci, Limerick, Ireland. [Singh, Ajay] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Singh, Ajay; Milliron, Delia J.] Univ Texas Austin, McKetta Dept Chem Engn, Austin, TX 78712 USA. RP Ryan, KM (reprint author), Univ Limerick, MSSI, Limerick, Ireland. EM Kevin.m.ryan@ul.ie RI Milliron, Delia/D-6002-2012; Ryan, kevin/D-8047-2011; Singh, Ajay/I-5538-2012; Foundry, Molecular/G-9968-2014 OI Ryan, kevin/0000-0003-3670-8505; Singh, Ajay/0000-0002-5168-7522; FU Science Foundation Ireland (SFI) under the Principal Investigator Program [11PI-1148]; U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported principally by Science Foundation Ireland (SFI) under the Principal Investigator Program (Contract No. 11PI-1148) and was conducted under the framework of the Irish Government's Programme for Research in Third Level Institutions Cycle 5, National Development Plan 2007-2013, with the assistance of the European Regional Development Fund. The authors acknowledge Fathima Laffir for XPS measurements. Some TEM and EDS mapping was carried out as a user project at The Molecular Foundry, supported under contract DE-AC02-05CH11231 from the U.S. Department of Energy. NR 60 TC 10 Z9 10 U1 7 U2 44 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD MAR 10 PY 2015 VL 27 IS 5 BP 1517 EP 1523 DI 10.1021/cm5035613 PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CD2ON UT WOS:000350919000010 ER PT J AU Niu, KY Lin, F Fang, L Nordlund, D Tao, RZ Weng, TC Doeff, MM Zheng, HM AF Niu, Kai-Yang Lin, Feng Fang, Liang Nordlund, Dennis Tao, Runzhe Weng, Tsu-Chien Doeff, Marca M. Zheng, Haimei TI Structural and Chemical Evolution of Amorphous Nickel Iron Complex Hydroxide upon Lithiation/Delithiation SO CHEMISTRY OF MATERIALS LA English DT Article ID LITHIUM-ION BATTERIES; SOLID-ELECTROLYTE INTERPHASE; TRANSITION-METAL OXIDES; SOFT-X-RAY; ANODE MATERIAL; CONVERSION; GRAPHENE; SPECTROSCOPY; PERFORMANCE; CAPACITY AB Development of novel electrode materials is essential to achieve high-performance lithium ion batteries. Here, we demonstrate that amorphous nickel iron complex hydroxides (Ni-Fe-OH) synthesized by a laser-chemical method can be used as a potential conversion anode material for lithium storage. Complementary characterizations, including ensemble-averaged X-ray absorption spectroscopy, spatially resolved electron energy-loss spectroscopy, and energy dispersive X-ray spectroscopy in a scanning transmission electron microscope, were performed to reveal the chemical and structural evolutions of the active hydroxide particles undergoing electrochemical cycling. The solid-electrolyte interphase (SEI) layer with a primary component of lithium fluoride (LiF) was found and remained robust on the particle surface during the charge/discharge processes, which suggests that the LiF-containing SEI layer plays a critical role in maintaining the stable capacity retention and good reversibility of the Ni-Fe-OH anode. C1 [Niu, Kai-Yang; Fang, Liang; Tao, Runzhe; Doeff, Marca M.; Zheng, Haimei] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA. [Lin, Feng] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Fang, Liang] Chongqing Univ, Coll Phys, State Key Lab Mech Transmiss, Chongqing 400044, Peoples R China. [Nordlund, Dennis; Weng, Tsu-Chien] SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94025 USA. [Zheng, Haimei] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. RP Zheng, HM (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA. EM hmzheng@lbl.gov RI Niu, Kaiyang/M-4765-2013; Nordlund, Dennis/A-8902-2008; OI Niu, Kaiyang/0000-0003-3289-1322; Nordlund, Dennis/0000-0001-9524-6908; Doeff, Marca/0000-0002-2148-8047 FU U.S. Department of Energy Office of Basic Energy Sciences [DE-AC02-05CH11231]; National Basic Research Program of China [2014CB931700]; NSFC [11074314, 11304405]; China Scholarship Council (CSC) [2010850533]; DOE Office of Science Early Career Research Program FX We used Tecnai and TitanX microscopes for structural analysis at the National Center for Electron Microscopy of Lawrence Berkeley National Laboratory (LBNL), which is supported by the U.S. Department of Energy Office of Basic Energy Sciences under Contract No. DE-AC02-05CH11231. The synchrotron X-ray portions of this research were carried out at the Stanford Synchrotron Radiation Lightsource (Beamlines 10-1 and 8-2), a directorate of SLAC National Accelerator Laboratory and an Office of Science User Facility operated for the U.S. Department of Energy Office of Science by Stanford University. L.F. acknowledges the support of the National Basic Research Program of China (2014CB931700), NSFC (Nos. 11074314, 11304405), and China Scholarship Council (CSC) under No. 2010850533. F.L., D.N., and T.-C.W. thank Dr. Jun-Sik Lee and Glen Kerr for the help at SSRL Beamline 8-2. H.Z. acknowledges the SinBeRise program of BEARS at University of California, Berkeley for travel support and the support of DOE Office of Science Early Career Research Program. NR 40 TC 3 Z9 3 U1 6 U2 68 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD MAR 10 PY 2015 VL 27 IS 5 BP 1583 EP 1589 DI 10.1021/cm5041375 PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CD2ON UT WOS:000350919000018 ER PT J AU Chatman, S Pearce, CI Rosso, KM AF Chatman, Shawn Pearce, Carolyn I. Rosso, Kevin M. TI Charge Transport at Ti-Doped Hematite (001)/Aqueous Interfaces SO CHEMISTRY OF MATERIALS LA English DT Article ID ALPHA-FE2O3 CRYSTAL FACES; BULK ELECTRONIC STATES; IRON-OXIDE ELECTRODES; FE2O3 SINGLE-CRYSTALS; ALPHA FERRIC OXIDE; ELECTRICAL-PROPERTIES; SEMICONDUCTOR ELECTRODES; WATER OXIDATION; THIN-FILMS; COMPUTER-SIMULATION AB Solid-state transport and electrochemical properties of Ti-doped hematite (alpha-(TixFe1-x)(2)O-3 (001) epitaxial thin films (x = 0.15, 0.21, and 0.42) were probed to achieve a better understanding of doped hematite for photoelectrochemical (PEC) applications. Room temperature resistivity measurements predict a resistivity minimum near x = 0.25 Ti doping, which can be rationalized as maximizing charge compensating Fe2+ concentration and Fe3+ electron accepting percolation pathways simultaneously. Temperature dependent resistivity data are consistent with small polaron hopping, revealing an activation energy that is Ti concentration dependent and commensurate with previously reported values (approximate to 0.11 eV). In contact with inert electrolyte, linear MottSchottky data at various pH values indicate that there is predominantly a single donor for Ti-doped hematite at x = 0.15 and x = 0.42 Ti concentrations. Two slope MottSchottky data at pH extremes indicate the presence of a second donor or surface state in the x = 0.21 Ti-doped film, with an energy level approximate to 0.7 eV below the Fermi level. MottSchottky plots indicate pH and Ti concentration dependent flatband potentials of -0.2 to -0.9 V vs SHE, commensurate with previously reported data. Flatband potentials exhibited super-Nernstian pH dependence ranging from -69.1 to -101.0 mV/pH. Carrier concentration data indicate that the Fermi energy of the Ti-doped system is Ti concentration dependent, with a minimum of 0.15 eV near x = 0.25. These energy level data allow us to construct an energy band diagram for Ti-doped hematite electrode/electrolyte interfaces, and to determine a Ti-doping concentration that reduces bulk resistivity while also reducing the formation of surface states for these photoanodes. C1 [Chatman, Shawn; Pearce, Carolyn I.; Rosso, Kevin M.] Pacific NW Natl Lab, Phys Sci Div, Richland, WA 99354 USA. [Chatman, Shawn] CALTECH, Joint Ctr Artificial Photosynth, Pasadena, CA 91125 USA. [Pearce, Carolyn I.] Univ Manchester, Sch Chem, Manchester M13 9PL, Lancs, England. [Pearce, Carolyn I.] Univ Manchester, Dalton Nucl Inst, Manchester M13 9PL, Lancs, England. RP Chatman, S (reprint author), Pacific NW Natl Lab, Phys Sci Div, Richland, WA 99354 USA. EM chatmans@caltech.edu; kevin.rosso@pnnl.gov FU Geosciences Research Program in the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences Biosciences FX This work was supported by the Geosciences Research Program in the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences & Biosciences. Portions of this research were performed using the Environmental Molecular Science Laboratory (EMSL) and the Advanced Light Source (ALS), both national scientific user facilities sponsored by the U.S. Department of Energy's Office of Biological and Environmental Research and Office of Basic Energy Sciences, respectively. EMSL is located at Pacific Northwest National Laboratory (PNNL), a multiprogram national laboratory operated for DOE by Battelle. We gratefully acknowledge the analytical assistance of Tim Droubay (MBE synthesis), Mark Engelhard (XPS), and Vaithiyalingam Shutthanandan (PIKE) at PNNL. NR 91 TC 6 Z9 6 U1 3 U2 84 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD MAR 10 PY 2015 VL 27 IS 5 BP 1665 EP 1673 DI 10.1021/cm504451j PG 9 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CD2ON UT WOS:000350919000028 ER PT J AU Haynes, AS Saouma, FO Otieno, CO Clark, DJ Shoemaker, DP Jang, JI Kanatzidis, MG AF Haynes, Alyssa S. Saouma, Felix O. Otieno, Calford O. Clark, Daniel J. Shoemaker, Daniel P. Jang, Joon I. Kanatzidis, Mercouri G. TI Phase-Change Behavior and Nonlinear Optical Second and Third Harmonic Generation of the One-Dimensional K(l-x)CsXPSe6 and Metastable beta-CsPSe6 SO CHEMISTRY OF MATERIALS LA English DT Article ID STRONG 2ND-HARMONIC GENERATION; DIRECT-BAND-GAP; GLASS-FIBERS; RB; SEMICONDUCTORS; CHALCOGENIDES; PHOSPHORUS; POLYMER; SALTS; GE AB The APSe(6) (A = K, K(1-x)Csx, Cs) family of one-dimensional (1D) materials was studied to examine the effects of the cation size on the nonlinear optical (NLO) response. The family has high-performing NLO properties with the noncentrosymmetric parent material, KPSe6, having infinite 1D chains of 1/(infinity)[PSe6-]. This structure has been successfully substituted with cesium up to K0.6Cs0.4PSe6 while retaining the polar character. All compounds crystallize in the space group Pca2(1) and have band gaps of 2.1 eV. In situ powder X-ray diffraction experiments using synchrotron radiation were used to determine the specifics of the amorphous to crystalline behavior and the crystallization and melting kinetics of the APSe(6) system. These measurements revealed a new phase, beta-CsPSe6, which is metastable and crystallizes in the noncentrosymmetric tetragonal space group P (4) over bar2(1)c with a = 12.526(2) angstrom, c = 12.781(3) angstrom, V = 2005.3(6) angstrom(3), and Z = 8. The structure is composed of 2 sets of mutually perpendicular 1/8[PSe6-] chains charge-balanced by Cs cations, and the band gap of beta-CsPSe6 is 1.9 eV. Second harmonic generation (SHG) measurements demonstrate that substitution of Cs into KPSe6 maintains the strong NLO signal with a very high SHG coefficient (chi((2))) of similar to 150 pm/V for K(1-x)CsxPSe6 and 30 pm/V for beta-CsPSe6. Laser-induced damage threshold analysis reveals APSe(6) exhibits two-photon absorption (2PA) at 1064 nm with input laser intensity greater than 1 GW/cm(2) and optical damage from 2PA at similar to 2 GW/cm(2). The materials also exhibit strong third harmonic generation (THG) with THG coefficients (chi((3)) x 10(5)) for KPSe6, K0.6Cs0.4PSe6, alpha-CsPSe6, and beta-CsPSe6 to be 2.6, 3.1, 1.8, and 1.1 pm(2)/V-2, respectively. C1 [Haynes, Alyssa S.; Kanatzidis, Mercouri G.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Saouma, Felix O.; Otieno, Calford O.; Clark, Daniel J.; Jang, Joon I.] SUNY Binghamton, Dept Phys Appl Phys & Astron, Binghamton, NY 13902 USA. [Shoemaker, Daniel P.; Kanatzidis, Mercouri G.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Shoemaker, Daniel P.] Univ Illinois, Dept Mat Sci & Engn, Urbana, IL 61801 USA. RP Kanatzidis, MG (reprint author), Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. EM m-kanatzidis@northwestern.edu OI Haynes, Alyssa/0000-0002-1268-0213 FU National Science Foundation [DMR-1410169]; U.S. DOE [DE-AC02-06CH11357]; State of Illinois; Northwestern University; National Science Foundation through the MRSEC program at the Materials Research Center [DMR-1121262]; National Science Foundation through The Nanoscale Science and Engineering Center [EEC-0118025/003]; National Science Foundation through a Graduate Research Fellowship [DGE-1324585] FX This work is supported by the National Science Foundation Grant DMR-1410169. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. This work also made use of the EPIC facility (NUANCE Center-Northwestern University), which has received support under the State of Illinois, Northwestern University, and the National Science Foundation with grants DMR-1121262 through the MRSEC program at the Materials Research Center, and EEC-0118025/003 through The Nanoscale Science and Engineering Center. The Raman experiments were performed in the IMSERC facility at Northwestern University and supported through the university. A.S.H. gratefully acknowledges support by the National Science Foundation through a Graduate Research Fellowship under Grant DGE-1324585. A.S.H. additionally appreciates the mentorship from Dr. Greg Halder, Dr. Christos D. Malliakas, Dr. Collin D. Morris, Dr. Amy Sarjeant, and Ms. Charlotte Stern that helped make this work possible. NR 53 TC 17 Z9 17 U1 6 U2 32 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD MAR 10 PY 2015 VL 27 IS 5 BP 1837 EP 1846 DI 10.1021/acs.chemmater.5b00065 PG 10 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CD2ON UT WOS:000350919000048 ER PT J AU Seaver, SMD Bradbury, LMT Frelin, O Zarecki, R Ruppin, E Hanson, AD Henry, CS AF Seaver, Samuel M. D. Bradbury, Louis M. T. Frelin, Oceane Zarecki, Raphy Ruppin, Eytan Hanson, Andrew D. Henry, Christopher S. TI Improved evidence-based genome-scale metabolic models for maize leaf, embryo, and endosperm SO FRONTIERS IN PLANT SCIENCE LA English DT Article DE systems biology; plant metabolism; transcriptomics; metabolic networks; flux balance analysis; Zea mays ID FLUX VARIABILITY ANALYSIS; STORAGE SYNTHESIS; PATHWAY DATABASE; BALANCE ANALYSIS; ACID SYNTHESIS; ARABIDOPSIS; RECONSTRUCTION; NETWORK; PLANTS; SEEDS AB There is a growing demand for genome-scale metabolic reconstructions for plants, fueled by the need to understand the metabolic basis of crop yield and by progress in genome and transcriptome sequencing. Methods are also required to enable the interpretation of plant transcriptome data to study how cellular metabolic activity varies under different growth conditions or even within different organs, tissues, and developmental stages. Such methods depend extensively on the accuracy with which genes have been mapped to the biochemical reactions in the plant metabolic pathways. Errors in these mappings lead to metabolic reconstructions with an inflated number of reactions and possible generation of unreliable metabolic phenotype predictions. Here we introduce a new evidence-based genome-scale metabolic reconstruction of maize, with significant improvements in the quality of the gene-reaction associations included within our model. We also present a new approach for applying our model to predict active metabolic genes based on transcriptome data. This method includes a minimal set of reactions associated with low expression genes to enable activity of a maximum number of reactions associated with high expression genes. We apply this method to construct an organ-specific model for the maize leaf, and tissue specific models for maize embryo and endosperm cells. We validate our models using fluxomics data for the endosperm and embryo, demonstrating an improved capacity of our models to fit the available fluxomics data. All models are publicly available via the DOE Systems Biology Knowledgebase and PlantSEED, and our new method is generally applicable for analysis transcript profiles from any plant, paving the way for further in silico studies with a wide variety of plant genomes. C1 [Seaver, Samuel M. D.; Henry, Christopher S.] Argonne Natl Lab, Div Math & Comp Sci, Argonne, IL 60439 USA. [Seaver, Samuel M. D.; Henry, Christopher S.] Univ Chicago, Computat Inst, Chicago, IL 60637 USA. [Bradbury, Louis M. T.; Frelin, Oceane; Hanson, Andrew D.] Univ Florida, Dept Hort Sci, Gainesville, FL USA. [Bradbury, Louis M. T.] CUNY, Dept Biol, York Coll, New York, NY 10021 USA. [Zarecki, Raphy; Ruppin, Eytan] Tel Aviv Univ, Sackler Fac Med, IL-69978 Tel Aviv, Israel. RP Henry, CS (reprint author), Argonne Natl Lab, Div Math & Comp Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM chrisshenry@gmail.com FU National Science Foundation [IOS-1025398]; C.V. Griffin Sr. Foundation; Office of Science, Office of Biological and Environmental Research, of the US Department of Energy [DE-ACO2-06CH11357]; DOE Systems Biology Knowledgebase FX This work was supported by National Science Foundation Grant Number IOS-1025398, by an endowment from the C.V. Griffin Sr. Foundation, and by the Office of Science, Office of Biological and Environmental Research, of the US Department of Energy under Contract Number DE-ACO2-06CH11357, as part of the DOE Systems Biology Knowledgebase. NR 86 TC 6 Z9 6 U1 2 U2 22 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-462X J9 FRONT PLANT SCI JI Front. Plant Sci. PD MAR 10 PY 2015 VL 6 AR 142 DI 10.3389/fpls2015.00142 PG 17 WC Plant Sciences SC Plant Sciences GA CD3IF UT WOS:000350971000001 PM 25806041 ER PT J AU Zhang, HH Liu, XP Feng, SR Wang, WJ Schmidt-Rohr, K Akinc, M Nilsen-Hamilton, M Vaknin, D Mallapragada, S AF Zhang, Honghu Liu, Xunpei Feng, Shuren Wang, Wenjie Schmidt-Rohr, Klaus Akinc, Mufit Nilsen-Hamilton, Marit Vaknin, David Mallapragada, Surya TI Morphological Transformations in the Magnetite Biomineralizing Protein Mms6 in Iron Solutions: A Small-Angle X-ray Scattering Study SO LANGMUIR LA English DT Article ID MAGNETOTACTIC BACTERIA; OXIDE NANOPARTICLES; NANOCRYSTALS; NANOSTRUCTURES; NANOSCALE; CRYSTAL; BIOLOGY; SYSTEMS; MODEL AB Magnetotactic bacteria that produce magnetic nanocrystals of uniform size and well-defined morphologies have inspired the use of biomineralization protein Mms6 to promote formation of uniform magnetic nanocrystals in vitro. Small angle X-ray scattering (SAXS) studies in physiological solutions reveal that Mms6 forms compact globular three-dimensional (3D) micelles (approximately 10 nm in diameter) that are, to a large extent, independent of concentration. In the presence of iron ions in the solutions, the general micellar morphology is preserved, however, with associations among micelles that are induced by iron ions. Compared with Mms6, the m2Mms6 mutant (with the sequence of hydroxyl/carboxyl containing residues in the C-terminal domain shuffled) exhibits subtle morphological changes in the presence of iron ions in solutions. The analysis of the SAXS data is consistent with a hierarchical core-corona micellar structure similar to that found in amphiphilic polymers. The addition of ferric and ferrous iron ions to the protein solution induces morphological changes in the micellar structure by transforming the 3D micelles into objects of reduced dimensionality of 2, with fractal-like characteristics (including Gaussian-chain-like) or, alternatively, platelet-like structures. C1 [Zhang, Honghu; Liu, Xunpei; Feng, Shuren; Wang, Wenjie; Schmidt-Rohr, Klaus; Akinc, Mufit; Nilsen-Hamilton, Marit; Vaknin, David; Mallapragada, Surya] US DOE, Ames Lab, Div Mat Sci & Engn, Ames, IA 50011 USA. [Zhang, Honghu; Akinc, Mufit] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. [Mallapragada, Surya] Iowa State Univ, Dept Chem & Biol Engn, Ames, IA 50011 USA. [Feng, Shuren; Nilsen-Hamilton, Marit] Iowa State Univ, Roy J Carver Dept Biochem Biophys & Mol Biol, Ames, IA 50011 USA. [Schmidt-Rohr, Klaus] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. [Vaknin, David] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. RP Wang, WJ (reprint author), US DOE, Ames Lab, Div Mat Sci & Engn, Ames, IA 50011 USA. EM wwang@ameslab.gov; suryakm@iastate.edu RI Vaknin, David/B-3302-2009 OI Vaknin, David/0000-0002-0899-9248 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; U.S. Department of Energy by Iowa State University [DE-AC02-07CH11358]; U.S. DOE [DE-AC02-06CH11357] FX We thank Xiaobin Zuo at beamline 12ID-B and Benjamin Reinhart at beamline 12BM-B of APS for technical support in SAXS. We thank Pierre E. Palo (Ames Laboratory) for kindly preparing the proteins. Research supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. Ames Laboratory is operated for the U.S. Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. NR 38 TC 13 Z9 13 U1 3 U2 32 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0743-7463 J9 LANGMUIR JI Langmuir PD MAR 10 PY 2015 VL 31 IS 9 BP 2818 EP 2825 DI 10.1021/la5044377 PG 8 WC Chemistry, Multidisciplinary; Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CD2OI UT WOS:000350918500025 PM 25669122 ER PT J AU Singh, S Junghans, A Watkins, E Kapoor, Y Toomey, R Majewski, J AF Singh, Saurabh Junghans, Ann Watkins, Erik Kapoor, Yash Toomey, Ryan Majewski, Jaroslaw TI Effects of Fluid Shear Stress on Polyelectrolyte Multi layers by Neutron Scattering Studies SO LANGMUIR LA English DT Article ID RAY REFLECTIVITY DATA; LEAST-SQUARES METHODS; PRECORNEAL TEAR FILM; MULTILAYERS; THICKNESS; CELL AB The structure of layer-by-layer (LbL) deposited nanofilm coatings consists of alternating polyethylenimine (PEI) and polystyrenesulfonate (PSS) films deposited on a single crystal quartz substrate. LbL-deposited nanofilms were investigated by neutron reflectomery (NR) in contact with water in the static and fluid shear stress conditions. The fluid shear stress was applied through a laminar flow of the liquid parallel to the quartz/polymer interface in a custom-built solid-liquid interface cell. The scattering length density profiles obtained from NR results of these polyelectrolyte multilayers (PEM), measured under different shear conditions, showed proportional decrease of volume fraction of water hydrating the polymers. For the highest shear rate applied (ca. 6800 s(-1)) the water volume fraction decreased by approximately 7%. The decrease of the volume fraction of water was homogeneous through the thickness of the film. Since there were not any significant changes in the total polymer thickness, it resulted in negative osmotic pressures in the film. The PEM films were compared with the behavior of thin films of thermoresponsive poly(N-isopropylacrylamide) (pNIPAM) deposited via spin-coating. The PEM and pNIPAM differ in their interactions with water molecules, and they showed opposite behaviors under the fluid shear stress. In both cases the polymer hydration was reversible upon the restoration of static conditions. A theoretical explanation is given to explain this difference in the effect of shear on hydration of polymeric thin films. C1 [Singh, Saurabh; Junghans, Ann; Watkins, Erik; Majewski, Jaroslaw] Los Alamos Natl Lab, Manuel Lujan Jr Neutron Scattering Ctr, MPA, Los Alamos, NM 87545 USA. [Kapoor, Yash] Vis Care R&D, Johns Creek, GA 30097 USA. [Toomey, Ryan] Univ S Florida, Dept Chem & Biomed Engn, Tampa, FL 33620 USA. RP Majewski, J (reprint author), Los Alamos Natl Lab, Manuel Lujan Jr Neutron Scattering Ctr, MPA, Los Alamos, NM 87545 USA. EM jarek@lanl.gov RI Junghans, Ann/A-4257-2011 OI Junghans, Ann/0000-0001-7061-4663 FU DOE Office of Basic Energy Sciences and Los Alamos National Laboratory under DOE [DE-AC52-06NA25396] FX This work benefited from the use of the Lujan Neutron Scattering Center at Los Alamos Neutron Science Center funded by the DOE Office of Basic Energy Sciences and Los Alamos National Laboratory under DOE Contract DE-AC52-06NA25396. We express special thanks to Flow Science, Inc., for providing the numerical flow simulation results and Dr. A. Zubelewicz (Los Alamos National Laboratory) for helpful discussions. NR 32 TC 3 Z9 3 U1 2 U2 20 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0743-7463 J9 LANGMUIR JI Langmuir PD MAR 10 PY 2015 VL 31 IS 9 BP 2870 EP 2878 DI 10.1021/acs.langmuir5b00037 PG 9 WC Chemistry, Multidisciplinary; Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA CD2OI UT WOS:000350918500031 PM 25689755 ER PT J AU Yamaguchi, H Badenes, C Foster, AR Bravo, E Williams, BJ Maeda, K Nobukawa, M Eriksen, KA Brickhouse, NS Petre, R Koyama, K AF Yamaguchi, Hiroya Badenes, Carles Foster, Adam R. Bravo, Eduardo Williams, Brian J. Maeda, Keiichi Nobukawa, Masayoshi Eriksen, Kristoffer A. Brickhouse, Nancy S. Petre, Robert Koyama, Katsuji TI A CHANDRASEKHAR MASS PROGENITOR FOR THE TYPE Ia SUPERNOVA REMNANT 3C 397 FROM THE ENHANCED ABUNDANCES OF NICKEL AND MANGANESE SO ASTROPHYSICAL JOURNAL LETTERS LA English DT Article DE atomic data; infrared: ISM; ISM: individual objects (3C 397, G41.1-0.3); ISM: supernova remnants; nuclear reactions, nucleosynthesis, abundances; X-rays: ISM ID DELAYED-DETONATION MODELS; LARGE-MAGELLANIC-CLOUD; X-RAY; CIRCUMSTELLAR MATERIAL; KEPLERS SUPERNOVA; WHITE-DWARFS; MILKY-WAY; NUCLEOSYNTHESIS; EMISSION; SPECTRA AB Despite decades of intense efforts, many fundamental aspects of Type Ia supernovae (SNe Ia) remain elusive. One of the major open questions is whether the mass of an exploding white dwarf (WD) is close to the Chandrasekhar limit. Here, we report the detection of strong K-shell emission from stable Fe-peak elements in the Suzaku X-ray spectrum of the Type Ia supernova remnant (SNR) 3C 397. The high Ni/Fe and Mn/Fe mass ratios (0.11-0.24 and 0.018-0.033, respectively) in the hot plasma component that dominates the K-shell emission lines indicate a degree of neutronization in the supernova ejecta that can only be achieved by electron capture in the dense cores of exploding WDs with a near-Chandrasekhar mass. This suggests a single-degenerate origin for 3C 397, since Chandrasekhar mass progenitors are expected naturally if the WD accretes mass slowly from a companion. Together with other results supporting the double-degenerate scenario, our work adds to the mounting evidence that both progenitor channels make a significant contribution to the SN Ia rate in star-forming galaxies. C1 [Yamaguchi, Hiroya; Williams, Brian J.; Petre, Robert] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Yamaguchi, Hiroya] Univ Maryland, Dept Astron, College Pk, MD 20742 USA. [Yamaguchi, Hiroya; Brickhouse, Nancy S.] Harvard Smithsonian Ctr Astrophys, Cambridge, MA 02138 USA. [Badenes, Carles] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Badenes, Carles] Univ Pittsburgh, Pittsburgh Particle Phys Astrophys & Cosmol Ctr P, Pittsburgh, PA 15260 USA. [Bravo, Eduardo] Univ Politecn Cataluna, ETS Arquitectura Valles, E-08173 Sant Cugat Del Valles, Spain. [Maeda, Keiichi] Kyoto Univ, Dept Astron, Sakyo Ku, Kyoto 6068502, Japan. [Maeda, Keiichi] Univ Tokyo, Kavli Inst Phys & Math Universe WPI, Kashiwa, Chiba 2778583, Japan. [Nobukawa, Masayoshi; Koyama, Katsuji] Kyoto Univ, Dept Phys, Sakyo Ku, Kyoto 6068502, Japan. [Eriksen, Kristoffer A.] Los Alamos Natl Lab, Theoret Design Div, Los Alamos, NM 87545 USA. [Koyama, Katsuji] Osaka Univ, Dept Earth & Space Sci, Toyonaka, Osaka 5600043, Japan. RP Yamaguchi, H (reprint author), NASA, Goddard Space Flight Ctr, Code 662, Greenbelt, MD 20771 USA. EM hiroya.yamaguchi@nasa.gov RI XRAY, SUZAKU/A-1808-2009; OI Brickhouse, Nancy/0000-0002-8704-4473; Bravo, Eduardo/0000-0003-0894-6450; Badenes, Carles/0000-0003-3494-343X FU Spanish MINECO [AYA2013-40545]; JSPS [23740141/26800100, 24740123, 23000004/24540229] FX We thank Drs. Ken'ichi Nomoto, Samar Safi- Harb, Randall K. Smith, and Michael C. Witthoeft for helpful discussion and suggestions. E.B. is supported by Spanish MINECO grant AYA2013-40545. Japanese authors acknowledge financial support by JSPS Grant-in-Aid for Scientific Research Numbers 23740141/26800100 (K.M.), 24740123 (M.N.), and 23000004/24540229 (K.K). NR 46 TC 21 Z9 21 U1 1 U2 4 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 2041-8205 EI 2041-8213 J9 ASTROPHYS J LETT JI Astrophys. J. Lett. PD MAR 10 PY 2015 VL 801 IS 2 AR L31 DI 10.1088/2041-8205/801/2/L31 PG 6 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA CD3NJ UT WOS:000350985200012 ER PT J AU Chen, Q Luan, ZJ Cheng, XL Xu, JH AF Chen, Qi Luan, Zheng-Jiao Cheng, Xiaolin Xu, Jian-He TI Molecular Dynamics Investigation of the Substrate Binding Mechanism in Carboxylesterase SO BIOCHEMISTRY LA English DT Article ID SITE-DIRECTED MUTAGENESIS; ALPHA-HYDROXY ACIDS; RESOLUTION; ESTERASES; SPECIFICITY; STABILITY; PACKAGE; FAMILY AB A recombinant carboxylesterase, cloned from Pseudomonas putida and designated as rPPE, is capable of catalyzing the bioresolution of racemic 2-acetoxy-2-(2'-chlorophenyl)acetate (rac-AcO-CPA) with excellent (S)-enantioselectivity. Semirational design of the enzyme showed that the W187H variant could increase the activity by similar to 100-fold compared to the wild type (WT) enzyme. In this study, we performed all-atom molecular dynamics (MD) simulations of both apo-rPPE and rPPE in complex with (S)-AcO-CPA to gain insights into the origin of the increased catalysis in the W187H mutant. Our results show differential binding of (S)-AcO-CPA in the WT and W187H enzymes, especially the interactions of the substrate with the two active site residues Ser159 and His286. The replacement of Trp187 by His leads to considerable structural rearrangement in the active site of W187H. Unlike in the WT rPPE, the cap domain in the W187 mutant shows an open conformation in the simulations of both apo and substrate-bound enzymes. This open conformation exposes the catalytic triad to the solvent through a water accessible channel, which may facilitate the entry of the substrate and/or the exit of the product. Binding free energy calculations confirmed that the substrate binds more strongly in W187H than in WT. On the basis of these computational results, we further predicted that the mutations W187Y and D287G might also be able to increase the substrate binding and thus improve the enzymes catalytic efficiency. Experimental binding and kinetic assays on W187Y and D287G show improved catalytic efficiency over WT, but not W187H. Contrary to our prediction, W187Y shows slightly decreased substrate binding coupled with a 100-fold increase in turnover rate, while in D287G the substrate binding is 8 times stronger but with a slightly reduced turnover rate. Our work provides important molecular-level insights into the binding of the (S)-AcO-CPA substrate to carboxylesterase rPPEs, which will help guide future development of more efficient rPPE variants. C1 [Chen, Qi; Luan, Zheng-Jiao; Xu, Jian-He] East China Univ Sci, State Key Lab Bioreactor Engn, Technol, Shanghai 200237, Peoples R China. [Cheng, Xiaolin] Oak Ridge Natl Lab, UT ORNL Ctr Mol Biophys, Oak Ridge, TN 37831 USA. [Cheng, Xiaolin] Univ Tennessee, Dept Biochem & Cellular & Mol Biol, Knoxville, TN 37996 USA. [Xu, Jian-He] E China Univ Sci & Technol, Shanghai Collaborat Innovat Ctr Biomfg, Shanghai 200237, Peoples R China. RP Cheng, XL (reprint author), Oak Ridge Natl Lab, UT ORNL Ctr Mol Biophys, Oak Ridge, TN 37831 USA. EM chengx@ornl.gov; jianhexu@ecust.edu.cn FU Postdoctoral Science Foundation of China [2014M551349]; National Natural Science Foundation of China [21276082]; Ministry of Science and Technology, China [2011CB710800, 2011AA02A210]; China National Special Fund for State Key Laboratory of Bioreactor Engineering [2060204]; Computer Science and Mathematics Division at the Oak Ridge National Laboratory [De-AC05-00OR22725] FX This work is supported by the Postdoctoral Science Foundation of China (Grant No. 2014M551349), National Natural Science Foundation of China (No. 21276082), Ministry of Science and Technology, China (Nos. 2011CB710800 and 2011AA02A210), and China National Special Fund for State Key Laboratory of Bioreactor Engineering (No. 2060204). X.C. is partially supported by Computer Science and Mathematics Division at the Oak Ridge National Laboratory, which is managed by UT-Battelle, LLC under US DOE Contract No. De-AC05-00OR22725. NR 37 TC 8 Z9 9 U1 5 U2 31 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0006-2960 J9 BIOCHEMISTRY-US JI Biochemistry PD MAR 10 PY 2015 VL 54 IS 9 BP 1841 EP 1848 DI 10.1021/bi5015612 PG 8 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA CD2OR UT WOS:000350919400013 PM 25711934 ER PT J AU Wu, Q Yin, YF Sun, SW Zhang, XP Wan, N Bai, Y AF Wu, Qing Yin, Yanfeng Sun, Shuwei Zhang, Xiaoping Wan, Ning Bai, Ying TI Novel AlF3 surface modified spinel LiMn1.5Ni0.5O4 for lithium-ion batteries: performance characterization and mechanism exploration SO ELECTROCHIMICA ACTA LA English DT Article DE Spinel LiMn1.5Ni0.5O4 (LMNO); Surface modification; Cycling performance; Solid electrolyte interface (SEI); Lithium-ion batteries (LIBs) ID COATED LINI0.5MN1.5O4 SPINEL; CATHODE MATERIALS; ELECTROCHEMICAL PERFORMANCE; ELEVATED-TEMPERATURES; CYCLING EFFICIENCY; ETHYLENE CARBONATE; ELECTROLYTE; LICOO2; IMPROVEMENT; GRAPHITE AB Spinel LiMn1.5Ni0.5O4 (LMNO) cathode material synthesized by a sol-gel method is modified by different contents of AlF3 through simple chemical deposition. The effects of AlF3 coating on the structural and electrochemical properties of LMNO cathodes are investigated using X-ray diffraction (XRD), Raman spectroscopy, field emission scanning electron microscopy (FESEM), electrochemical impedance spectroscopy (EIS), Fourier transform infrared spectroscopy (FTIR) and differential scanning calorimetry (DSC). It is found that the AlF3 surface modification layers do not change the bulk structure of LMNO. Compared with the pristine sample, the AlF3-coated LMNO materials display enhanced cycling stabilities. Especially, the 1 wt% AlF3-coated LMNO demonstrates the best reversibility, with capacity retention of 93.6% after 50 cycles, much higher than that of the pristine material, 77.6%. EIS and FTIR data illustrate that the improvement of electrochemical performance can be attributed to the suppression of solid electrolyte interface (SEI) growth by AlF3 coating layer. DSC tests show that the AlF3 coating layer also helps in enhancing the thermal stability of LMNO cathode. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Wu, Qing; Yin, Yanfeng; Sun, Shuwei; Zhang, Xiaoping; Wan, Ning; Bai, Ying] Henan Univ, Key Lab Photovolta Mat Henan Prov, Kaifeng 475004, Peoples R China. [Wu, Qing; Yin, Yanfeng; Sun, Shuwei; Zhang, Xiaoping; Wan, Ning; Bai, Ying] Henan Univ, Sch Phys & Elect, Kaifeng 475004, Peoples R China. [Bai, Ying] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. RP Bai, Y (reprint author), Henan Univ, Key Lab Photovolta Mat Henan Prov, Kaifeng 475004, Peoples R China. EM ybai@henu.edu.cn FU National Natural Science Foundation of China [50902044]; Program for Innovative Research Team in Science and Technology in University of Henan Province (IRTSTHN) [2012IRTSTHN004]; Innovation Scientists and Technicians Troop Construction Projects of Henan Province [124200510004]; State Scholarship Fund from China Scholarship Council FX This work was supported by the National Natural Science Foundation of China (50902044), the Program for Innovative Research Team in Science and Technology in University of Henan Province (IRTSTHN) (2012IRTSTHN004), the Innovation Scientists and Technicians Troop Construction Projects of Henan Province (124200510004), and the State Scholarship Fund from China Scholarship Council. NR 45 TC 8 Z9 9 U1 14 U2 90 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0013-4686 EI 1873-3859 J9 ELECTROCHIM ACTA JI Electrochim. Acta PD MAR 10 PY 2015 VL 158 BP 73 EP 80 DI 10.1016/j.electacta.2015.01.145 PG 8 WC Electrochemistry SC Electrochemistry GA CC6AD UT WOS:000350446000011 ER PT J AU Chen, L Wu, G Holby, EF Zelenay, P Tao, WQ Kang, QJ AF Chen, Li Wu, Gang Holby, Edward F. Zelenay, Piotr Tao, Wen-Quan Kang, Qinjun TI Lattice Boltzmann Pore-Scale Investigation of Coupled Physical-electrochemical Processes in C/Pt and Non-Precious Metal Cathode Catalyst Layers in Proton Exchange Membrane Fuel Cells SO ELECTROCHIMICA ACTA LA English DT Article DE Proton exchange membrane fuel cell; catalyst layer; non-precious metal catalyst; reactive transport; effective transport properties; Lattice Boltzmann method ID DIRECT NUMERICAL-SIMULATION; EFFECTIVE TRANSPORT-PROPERTIES; OXYGEN REDUCTION REACTION; GAS-DIFFUSION; MICROSTRUCTURE RECONSTRUCTION; FINITE-VOLUME; MODEL; ELECTRODES; CARBON; PERFORMANCE AB High-resolution porous structures of catalyst layers (CLs) including non-precious metal catalysts (NPMCs) or Pt for proton exchange membrane fuel cells are reconstructed using the quartet structure generation set. The nanoscale structures are analyzed in terms of pore size distribution, specific surface area, and phase connectivity. Pore-scale simulation methods based on the lattice Boltzmann method are developed to predict the macroscopic transport properties in CLs. The non-uniform distribution of ionomer in CL generates more tortuous pathways for reactant transport, greatly reducing the effective diffusivity. The tortuosity of CLs is much higher than that adopted by the Bruggeman equation. Knudsen diffusion plays a significant role in oxygen diffusion and significantly reduces the effective diffusivity. Reactive transport inside the CLs is also investigated. Although the reactive surface area of the non-precious metal catalyst (NPMC) CL is much higher than that of the Pt CL, the oxygen reaction rate is lower in the NPMC CL due to the much lower reaction rate coefficient. Although pores of a few nanometers in size can increase the number of reactive sites in NPMC CLs, they contribute little to enhance the mass transport. Mesopores, which are a few tens of nanometers or larger in size, are shown to be required in order to increase the mass transport rate. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Chen, Li; Tao, Wen-Quan] Xi An Jiao Tong Univ, Sch Energy & Power Engn, Key Lab Thermo Fluid Sci & Engn MOE, Xian 710049, Shaanxi, Peoples R China. [Chen, Li; Kang, Qinjun] Los Alamos Natl Lab, Earth & Environm Sci Div, Los Alamos, NM USA. [Wu, Gang; Zelenay, Piotr] Los Alamos Natl Lab, Mat Phys & Applicat Div, Los Alamos, NM USA. [Holby, Edward F.] Los Alamos Natl Lab, Mat Sci & Technol Div, Los Alamos, NM USA. RP Kang, QJ (reprint author), Los Alamos Natl Lab, Earth & Environm Sci Div, Los Alamos, NM USA. RI Chen, Li/P-4886-2014; Wu, Gang/E-8536-2010; Kang, Qinjun/A-2585-2010; OI Chen, Li/0000-0001-7956-3532; Wu, Gang/0000-0003-4956-5208; Kang, Qinjun/0000-0002-4754-2240; Holby, Edward/0000-0001-8419-6298 FU LANL's LDRD Program; Institutional Computing Program; National Nature Science Foundation of China [51406145, 51136004, 51320105004]; China Postdoctoral Science Foundation [2014M550496] FX The authors acknowledge the support of LANL's LDRD Program, Institutional Computing Program, National Nature Science Foundation of China (51406145, 51136004 and 51320105004), and China Postdoctoral Science Foundation (2014M550496). Li Chen appreciates the helpful discussions with Doctor Yutong Mu and WenZhen Fang from Xi'an Jiaotong University, China, and Prof. Gregory A. Voth from the University of Chicago, USA. NR 59 TC 18 Z9 18 U1 9 U2 81 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0013-4686 EI 1873-3859 J9 ELECTROCHIM ACTA JI Electrochim. Acta PD MAR 10 PY 2015 VL 158 BP 175 EP 186 DI 10.1016/j.electacta.2015.01.121 PG 12 WC Electrochemistry SC Electrochemistry GA CC6AD UT WOS:000350446000023 ER PT J AU Raftopoulos, KN Koutsoumpis, S Jancia, M Lewicki, JP Kyriakos, K Mason, HE Harley, SJ Hebda, E Papadakis, CM Pielichowski, K Pissis, P AF Raftopoulos, Konstantinos N. Koutsoumpis, Stefanos Jancia, Malgorzata Lewicki, James P. Kyriakos, Konstantinos Mason, Harris E. Harley, Stephen J. Hebda, Edyta Papadakis, Christine M. Pielichowski, Krzysztof Pissis, Polycarpos TI Reduced Phase Separation and Slowing of Dynamics in Polyurethanes with Three-Dimensional POSS-Based Cross-Linking Moieties SO MACROMOLECULES LA English DT Article ID POLYHEDRAL OLIGOMERIC SILSESQUIOXANE; GLASS-TRANSITION TEMPERATURE; MOLECULAR-DYNAMICS; BLOCK-COPOLYMERS; SEGMENTED POLYURETHANES; INTEGRAL-EQUATIONS; DIELECTRIC-RELAXATION; HARD-SEGMENT; POLYMERS; NANOCOMPOSITES AB Octa-OH-functional POSS has been incorporated into a model polyurethane elastomer as a comparatively massive and notionally "robust" 3-dimensional cross-linking core. The effects of this cross-linking moiety on the morphology and molecular dynamics of the system are studied over a range of size and time scales. Microscopy, scattering, spectroscopic, thermal, and dielectric techniques, in agreement with each other, show that the covalent inclusion of the cross-linking particles restricts microphase separation, inhibits the formation of hard-block domains, and decelerates the motional dynamics of the polyurethane backbone. The effects on both the morphology and the dynamics of the polyurethane system are not continuous but occur in a steplike manner in the loading region of 4-6 wt % POSS. This critical region is thought to correspond to a sterically induced transition from one dominant morphology (microphase segregated) to an increasingly homogeneous nanophase segregated domain morphology. Contrary to expectations, cross-linking, even by the presumably rigid siliceous nanoparticles, reduces the mechanical modulus. In conjunction with the reduction of microphase separation, this observation indicates that the hard microdomains reinforce the polymer more effectively than the chemical cross-links. C1 [Raftopoulos, Konstantinos N.; Jancia, Malgorzata; Kyriakos, Konstantinos; Hebda, Edyta; Papadakis, Christine M.; Pielichowski, Krzysztof] Cracow Univ Technol, Dept Chem & Technol Polymers, PL-31155 Krakow, Poland. [Koutsoumpis, Stefanos; Pissis, Polycarpos] Natl Tech Univ Athens, Dept Phys, Athens 15780, Greece. [Lewicki, James P.; Mason, Harris E.; Harley, Stephen J.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Raftopoulos, KN (reprint author), Tech Univ Munich, Phys Dept, Fachgebiet Phys Weicher Mat, James Franck Str 1, D-85748 Garching, Germany. EM konstantinos.raftopoulos@ph.tum.de RI Hebda, Edyta/F-7925-2015; Mason, Harris/F-7194-2011; Raftopoulos, Konstantinos/D-5065-2016 OI Mason, Harris/0000-0002-1840-0550; Raftopoulos, Konstantinos/0000-0002-3055-5598 FU National Science Center in Poland [DEC-2011/02/A/ST8/00409]; European Union (European Social Fund ESF); Greek national funds through the Operational Program Education and Lifelong Learning, Research Funding Programs Aristeia and Thales; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX The authors gratefully acknowledge technical assistance with DMA measurements by Dr. Joanna Pagacz (CUT). The analysis of dielectric and X-ray data was performed with the software grafity, created and maintained by Dr. Daniel Fragiadakis. This work has been cofunded by the National Science Center in Poland under Contract No. DEC-2011/02/A/ST8/00409 (K.N.R., E.H., M.J., and K.P.). This research has been cofinanced by the European Union (European Social Fund ESF) and Greek national funds through the Operational Program Education and Lifelong Learning, Research Funding Programs Aristeia and Thales (S.K. and P.P.). Portions of this work were performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344 (J.P.L., H.E.M., and S.J.H.). The final version of this manuscript was formed during S.K.'s COST MP1105-17395 short term scientific mission (STSM) to CUT. NR 73 TC 14 Z9 14 U1 10 U2 76 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD MAR 10 PY 2015 VL 48 IS 5 BP 1429 EP 1441 DI 10.1021/ma5023132 PG 13 WC Polymer Science SC Polymer Science GA CD2OK UT WOS:000350918700021 ER PT J AU Mattsson, AE Rider, WJ AF Mattsson, Ann E. Rider, W. J. TI Artificial viscosity: back to the basics SO INTERNATIONAL JOURNAL FOR NUMERICAL METHODS IN FLUIDS LA English DT Article DE artificial viscosity; Hugoniot; Rayleigh line; Robert Richtmyer; John von Neumann; dissipation ID HYPERBOLIC CONSERVATION-LAWS; CENTERED LAGRANGIAN SCHEME; COMPRESSIBLE FLOW PROBLEMS; HIGH-RESOLUTION SCHEMES; HYDRODYNAMICS ALGORITHM; DIFFERENCE SCHEME; GODUNOV SCHEME; SOLVER; FLUX; COMPUTATIONS AB In this paper, we take a different perspective on the derivation of artificial viscosity. Heretofore, the development of artificial viscosity has been based on the paper published in Journal of Applied Physics in 1950 authored by John von Neumann and Robert Richtmyer [1]. Earlier, in 1948, Richtmyer published a report at Los Alamos Scientific Laboratory documenting the original concept [2]. This report was the true origin of shock capturing methods and contains several key ideas that are conceptually different than the 1950 journal article. Unfortunately, this report (LA-671) was classified until 1993. This has resulted in two issues: the misattribution of the invention of artificial viscosity as primarily being the work of von Neumann and the loss of the structurally different ideas in the original report. We seek to right the record of history here and use the ideas contained in Richtmyer's report to good effect in deriving a new shock viscosity. The focus of previous development has been the Hugoniot curve describing the locus of states connected by a single shock wave. Here we follow a path more focused upon the Rayleigh line, which is strongly guided by Richtmyer's line of development of the original artificial viscosity formulation. We provide an implementation of the method resulting from this perspective and computational results for simple shock problems. Copyright (C) 2014 John Wiley & Sons, Ltd. C1 [Mattsson, Ann E.; Rider, W. J.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Mattsson, AE (reprint author), Sandia Natl Labs, Dept 1444, Mail Stop 1322, Albuquerque, NM 87185 USA. EM aematts@sandia.gov NR 67 TC 1 Z9 1 U1 2 U2 19 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0271-2091 EI 1097-0363 J9 INT J NUMER METH FL JI Int. J. Numer. Methods Fluids PD MAR 10 PY 2015 VL 77 IS 7 BP 400 EP 417 DI 10.1002/fld.3981 PG 18 WC Computer Science, Interdisciplinary Applications; Mathematics, Interdisciplinary Applications; Mechanics; Physics, Fluids & Plasmas SC Computer Science; Mathematics; Mechanics; Physics GA CB8QY UT WOS:000349897000002 ER PT J AU Wright, AV Sternberg, SH Taylor, DW Staahl, BT Bardales, JA Kornfeld, JE Doudna, JA AF Wright, Addison V. Sternberg, Samuel H. Taylor, David W. Staahl, Brett T. Bardales, Jorge A. Kornfeld, Jack E. Doudna, Jennifer A. TI Rational design of a split-Cas9 enzyme complex SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE CRISPR-Cas9; genome engineering; split enzyme ID GUIDED SURVEILLANCE COMPLEX; CRISPR-CAS SYSTEMS; CRYSTAL-STRUCTURE; PROTEIN INTERACTIONS; ESCHERICHIA-COLI; TARGET DNA; RNA; IMMUNITY; CELLS; ENDONUCLEASE AB Cas9, an RNA-guided DNA endonuclease found in clustered regularly interspaced short palindromic repeats (CRISPR) bacterial immune systems, is a versatile tool for genome editing, transcriptional regulation, and cellular imaging applications. Structures of Streptococcus pyogenes Cas9 alone or bound to single-guide RNA (sgRNA) and target DNA revealed a bilobed protein architecture that undergoes major conformational changes upon guide RNA and DNA binding. To investigate the molecular determinants and relevance of the interlobe rearrangement for target recognition and cleavage, we designed a split-Cas9 enzyme in which the nuclease lobe and a-helical lobe are expressed as separate polypeptides. Although the lobes do not interact on their own, the sgRNA recruits them into a ternary complex that recapitulates the activity of full-length Cas9 and catalyzes site-specific DNA cleavage. The use of a modified sgRNA abrogates split-Cas9 activity by preventing dimerization, allowing for the development of an inducible dimerization system. We propose that split-Cas9 can act as a highly regulatable platform for genome-engineering applications. C1 [Wright, Addison V.; Staahl, Brett T.; Kornfeld, Jack E.; Doudna, Jennifer A.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Sternberg, Samuel H.; Doudna, Jennifer A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Taylor, David W.; Doudna, Jennifer A.] Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA. [Bardales, Jorge A.; Doudna, Jennifer A.] Univ Calif Berkeley, Biophys Grad Grp, Berkeley, CA 94720 USA. [Doudna, Jennifer A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Doudna, JA (reprint author), Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. EM doudna@berkeley.edu OI Taylor, David/0000-0002-6198-1194 FU Howard Hughes Medical Institute; NIGMS NIH HHS [T32 GM007232, T32 GM066698] NR 26 TC 53 Z9 54 U1 8 U2 64 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAR 10 PY 2015 VL 112 IS 10 BP 2984 EP 2989 DI 10.1073/pnas.1501698112 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CC8VK UT WOS:000350646500035 PM 25713377 ER PT J AU Chowdhury, C Chun, S Pang, A Sawaya, MR Sinha, S Yeates, TO Bobik, TA AF Chowdhury, Chiranjit Chun, Sunny Pang, Allan Sawaya, Michael R. Sinha, Sharmistha Yeates, Todd O. Bobik, Thomas A. TI Selective molecular transport through the protein shell of a bacterial microcompartment organelle SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE microcompartment; protein channel; carboxysome; Salmonella; B-12 ID B-12-DEPENDENT 1,2-PROPANEDIOL DEGRADATION; SEROVAR TYPHIMURIUM LT2; SALMONELLA-ENTERICA; LACTOBACILLUS-REUTERI; CARBOXYSOME SHELL; ESCHERICHIA-COLI; ETHANOLAMINE; MECHANISMS; METABOLITE; GLYCEROL AB Bacterial microcompartments are widespread prokaryotic organelles that have important and diverse roles ranging from carbon fixation to enteric pathogenesis. Current models for microcompartment function propose that their outer protein shell is selectively permeable to small molecules, but whether a protein shell can mediate selective permeability and how this occurs are unresolved questions. Here, biochemical and physiological studies of structure-guided mutants are used to show that the hexameric PduA shell protein of the 1,2-propanediol utilization (Pdu) microcompartment forms a selectively permeable pore tailored for the influx of 1,2-propanediol (the substrate of the Pdu microcompartment) while restricting the efflux of propionaldehyde, a toxic intermediate of 1,2-propanediol catabolism. Crystal structures of various PduA mutants provide a foundation for interpreting the observed biochemical and phenotypic data in terms of molecular diffusion across the shell. Overall, these studies provide a basis for understanding a class of selectively permeable channels formed by nonmembrane proteins. C1 [Chowdhury, Chiranjit; Sinha, Sharmistha; Bobik, Thomas A.] Iowa State Univ, Roy J Carver Dept Biochem Biophys & Mol Biol, Ames, IA 50011 USA. [Chun, Sunny; Yeates, Todd O.] Univ Calif Los Angeles, Mol Biol Inst, Los Angeles, CA 90095 USA. [Pang, Allan; Sawaya, Michael R.; Yeates, Todd O.] Univ Calif Los Angeles, UCLA DOE Inst Genom & Prote, Los Angeles, CA 90095 USA. [Yeates, Todd O.] Univ Calif Los Angeles, Dept Chem & Biochem, Los Angeles, CA 90095 USA. RP Yeates, TO (reprint author), Univ Calif Los Angeles, Mol Biol Inst, Los Angeles, CA 90095 USA. EM yeates@mbi.ucla.edu; bobik@iastate.edu OI Sawaya, Michael/0000-0003-0874-9043; Yeates, Todd/0000-0001-5709-9839 FU National Center for Research Resources Grant [5P41RR015301-10]; National Institute of General Medical Sciences Grant from NIH [8 P41 GM103403-10]; NIH [R01AI081146]; Biological and Environmental Research program of the Department of Energy (DOE) Office of Science; Chemistry-Biology Interface NIH Training Grant [T32-GM008496]; University of California, Los Angeles Graduate Division; DOE [DE-AC02-06CH11357] FX We thank the Iowa State University nanoimaging and DNA sequencing and synthesis facilities for help with the electron microscopy and DNA sequencing, Michael Collazo and Duilio Cascio for assistance in protein crystallization and data collection, and the synchrotron staff at Advanced Photon Source (APS) Beamline 24-ID-C. We also thank M. Capel, K. Rajashankar, N. Sukumar, J. Schuermann, I. Kourinov, and F. Murphy (Northeastern Collaborative Access Team Beamline 24-ID-C at APS, which is supported by National Center for Research Resources Grant 5P41RR015301-10 and National Institute of General Medical Sciences Grant 8 P41 GM103403-10 from NIH). This work was supported by NIH Grant R01AI081146 (to T.O.Y. and T.A.B.). Work in the T.O.Y. laboratory was supported by the Biological and Environmental Research program of the Department of Energy (DOE) Office of Science. S.C. was supported by a Chemistry-Biology Interface NIH Training Grant T32-GM008496 and by the University of California, Los Angeles Graduate Division. Use of the APS is supported by the DOE under Contract DE-AC02-06CH11357. NR 36 TC 20 Z9 20 U1 9 U2 26 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAR 10 PY 2015 VL 112 IS 10 BP 2990 EP 2995 DI 10.1073/pnas.1423672112 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA CC8VK UT WOS:000350646500036 PM 25713376 ER PT J AU Vandiver, MA Caire, BR Poskin, Z Li, YF Seifert, S Knauss, DM Herring, AM Liberatore, MW AF Vandiver, Melissa A. Caire, Benjamin R. Poskin, Zach Li, Yifan Seifert, Soenke Knauss, Daniel M. Herring, Andrew M. Liberatore, Matthew W. TI Durability and Performance of Polystyrene-b-Poly(vinylbenzyl trimethylammonium) Diblock Copolymer and Equivalent Blend Anion Exchange Membranes SO JOURNAL OF APPLIED POLYMER SCIENCE LA English DT Article DE batteries and fuel cells; conducting polymers; copolymers; mechanical properties; membranes ID POLYMER ELECTROLYTE MEMBRANES; FUEL-CELL APPLICATIONS; MECHANICAL-PROPERTIES; TRANSPORT-PROPERTIES; BLOCK-COPOLYMERS; WATER-UPTAKE; CONDUCTIVITY; TEMPERATURE; HYDROXIDE; HYDRATION AB Anion exchange membranes (AEM) are solid polymer electrolytes that facilitate ion transport in fuel cells. In this study, a polystyrene-b-poly(vinylbenzyl trimethylammonium) diblock copolymer was evaluated as potential AEM and compared with the equivalent homopolymer blend. The diblock had a 92% conversion of reactive sites with an IEC of 1.72 +/- 0.05 mmol g(-1), while the blend had a 43% conversion for an IEC of 0.80 +/- 0.03 mmol g(-1). At 50 degrees C and 95% relative humidity, the chloride conductivity of the diblock was higher, 24-33 mS cm(-1), compared with the blend, 1-6 mS cm(-1). The diblock displayed phase separation on the length scale of 100 nm, while the blend displayed microphase separation (similar to 10 mu m). Mechanical characterization of films from 40 to 90 microns thick found that elasticity and elongation decreased with the addition of cations to the films. At humidified conditions, water acted as a plasticizer to increase film elasticity and elongation. While the polystyrene-based diblock displayed sufficient ionic conductivity, the films' mechanical properties require improvement, i.e., greater elasticity and strength, before use in fuel cells. (C) 2014 Wiley Periodicals, Inc. C1 [Vandiver, Melissa A.; Caire, Benjamin R.; Poskin, Zach; Herring, Andrew M.; Liberatore, Matthew W.] Colorado Sch Mines, Dept Chem & Biol Engn, Golden, CO 80401 USA. [Li, Yifan; Knauss, Daniel M.] Colorado Sch Mines, Dept Chem & Geochem, Golden, CO 80401 USA. [Seifert, Soenke] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. RP Liberatore, MW (reprint author), Colorado Sch Mines, Dept Chem & Biol Engn, Golden, CO 80401 USA. EM mliberat@mines.edu RI Liberatore, Matthew/B-6828-2008; OI Caire, Benjamin/0000-0003-3379-7733; Li, Yifan/0000-0002-9142-0232; Herring, Andrew/0000-0001-7318-5999 FU Army Research Office under MURI [W911NF-10-1-0520]; Army Research Office under DURIPs [W911NF-11-1-0306, W911NF-11-1-0462]; U.S. DOE [DE-AC02-06CH11357] FX The authors thank the Army Research Office for support of this research under the MURI #W911NF-10-1-0520 and DURIPs #W911NF-11-1-0306 and #W911NF-11-1-0462. Some measurements were completed as part of the NSF Polymer REU EEC-1156745. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. NR 47 TC 13 Z9 13 U1 11 U2 118 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0021-8995 EI 1097-4628 J9 J APPL POLYM SCI JI J. Appl. Polym. Sci. PD MAR 10 PY 2015 VL 132 IS 10 AR 41596 DI 10.1002/app.41596 PG 9 WC Polymer Science SC Polymer Science GA AW6DH UT WOS:000346359100024 ER PT J AU Markov, P Appavoo, K Haglund, RF Weiss, SM AF Markov, Petr Appavoo, Kannatassen Haglund, Richard F., Jr. Weiss, Sharon M. TI Hybrid Si-VO2-Au optical modulator based on near-field plasmonic coupling SO OPTICS EXPRESS LA English DT Article ID SILICON ELECTROOPTIC MODULATOR; TO-METAL TRANSITION; WAVE-GUIDE; SUBWAVELENGTH CONFINEMENT; PHASE-TRANSITION; COMPACT; VO2; OXIDE; SYSTEM; DRIVEN AB We present a computational design for an integrated electro-optic modulator based on near-field plasmonic coupling between gold nanodisks and a thin film of vanadium dioxide on a silicon substrate. Active modulation is achieved by applying a time-varying electric field to initiate large changes in the refractive index of vanadium dioxide. Significant decrease in device footprint (200 nm x 560 nm) and increase in extinction ratio per unit length (9 dB/mu m) compared to state-of-the-art photonic and plasmonic modulators are predicted. (C) 2015 Optical Society of America C1 [Markov, Petr; Weiss, Sharon M.] Vanderbilt Univ, Dept Elect Engn & Comp Sci, Nashville, TN 37235 USA. [Appavoo, Kannatassen; Haglund, Richard F., Jr.; Weiss, Sharon M.] Vanderbilt Univ, Interdisciplinary Grad Program Mat Sci, Nashville, TN 37235 USA. [Appavoo, Kannatassen] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Haglund, Richard F., Jr.; Weiss, Sharon M.] Vanderbilt Univ, Dept Phys & Astron, Nashville, TN 37235 USA. RP Markov, P (reprint author), Vanderbilt Univ, Dept Elect Engn & Comp Sci, Nashville, TN 37235 USA. EM petr.markov@vanderbilt.edu FU Air Force Office of Scientific Research [FA9550-10-1-0366]; U. S. Department of Energy, Office of Science [DE-FG01-02ER45916] FX PM and SMW acknowledge support from the Air Force Office of Scientific Research (FA9550-10-1-0366). KA was supported by the U. S. Department of Energy, Office of Science (DE-FG01-02ER45916) and contributed expertise on plasmonics and plasmonic coupling with vanadium dioxide. NR 48 TC 13 Z9 13 U1 4 U2 26 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD MAR 9 PY 2015 VL 23 IS 5 BP 6878 EP 6887 DI 10.1364/OE.23.006878 PG 10 WC Optics SC Optics GA CD2BL UT WOS:000350878500145 PM 25836907 ER PT J AU Aad, G Abbott, B Abdallah, J Khalek, SA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Agatonovic-Jovin, T Aguilar-Saavedra, JA Agustoni, M Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TPA Akimoto, G Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Allbrooke, BMM Allison, LJ Allport, PP Almond, J Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Anduaga, XS Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonaki, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Apolle, R Arabidze, G Aracena, I Arai, Y Araque, JP Arce, ATH Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Arnaez, O Arnal, V Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Asai, S Asbah, N Ashkenazi, A Asman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Auerbach, B Augsten, K Aurousseau, M Avolio, G Azuelos, G Azuma, Y Baak, MA Baas, A Bacci, C Bachacou, H Bachas, K Backes, M Backhaus, M Mayes, JB Badescu, E Bagiacchi, P Bagnaia, P Bai, Y Bain, T Baines, JT Baker, OK Balek, P Balli, F Banas, E Banerjee, S Bannoura, AAE Bansal, V Bansil, HS Barak, L Baranov, SP Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, P Bartsch, V Bassalat, A 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Blackburn, D Blair, RE Blanchard, JB Blazek, T Bloch, I Blocker, C Blum, W Blumenschein, U Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Bock, C Boddy, CR Boehler, M Boek, TT Bogaerts, JA Bogdanchikov, AG Bogouch, A Bohm, C Bohm, J Boisvert, V Bold, T Boldea, V Boldyrev, AS Bomben, M Bona, M Boonekamp, M Borisov, A Borissov, G Borri, M Borroni, S Bortfeldt, J Bortolotto, V Bos, K Boscherini, D Bosman, M Boterenbrood, H Boudreau, J Bouffard, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boutouil, S Boveia, A Boyd, J Boyko, IR Bracinik, J Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Brazzale, SF Brelier, B Brendlinger, K Brennan, AJ Brenner, R Bressler, S Bristow, K Bristow, TM Britton, D Brochu, FM Brock, I Brock, R Bromberg, C Bronner, J Brooijmans, G Brooks, T Brooks, WK Brosamer, J Brost, E Brown, J de Renstrom, PAB Bruncko, D Bruneliere, R Brunet, S Bruni, A Bruni, G Bruschi, M Bryngemark, L Buanes, T Buat, Q Bucci, F Buchholz, P 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CA ATLAS Collaboration TI Search for new phenomena in the dijet mass distribution using pp collision data at root s=8 TeV with the ATLAS detector SO PHYSICAL REVIEW D LA English DT Article ID PROTON-PROTON COLLISIONS; CARLO EVENT GENERATOR; BLACK-HOLE PRODUCTION; ANGULAR-DISTRIBUTIONS; PARTON DISTRIBUTIONS; HADRON COLLIDERS; STANDARD MODEL; CHIRAL COLOR; 1 FB(-1); BOSONS AB Dijet events produced in LHC proton-proton collisions at a center-of-mass energy root s = 8 TeV are studied with the ATLAS detector using the full 2012 data set, with an integrated luminosity of 20.3 fb(-1). Dijet masses up to about 4.5 TeV are probed. No resonancelike features are observed in the dijet mass spectrum. Limits on the cross section times acceptance are set at the 95% credibility level for various hypotheses of new phenomena in terms of mass or energy scale, as appropriate. 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[Otero y Garzon, G.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Buttinger, W.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Frost, J. A.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Robinson, D.; Sandoval, T.; Thomson, M.; Ward, C. P.; Williams, S.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Leight, W. A.; Marchand, J. F.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Abreu, R.; Aleksa, M.; Andari, N.; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Battistin, M.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Dell'Acqua, A.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duehrssen, M.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Perez, S. Fernandez; Franchino, S.; Francis, D.; Froidevaux, D.; Garonne, V.; Gianotti, F.; Gillberg, D.; Glatzer, J.; Godlewski, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hauschild, M.; Hawkings, R. J.; Heller, M.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Hubacek, Z.; Huhtinen, M.; Jaekel, M. R.; Jakobsen, S.; Jansen, H.; Jenni, P.; Jungst, R. M.; Kaneda, M.; Klioutchnikova, T.; Krasznahorkay, A.; Lantzsch, K.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Martin, B.; Marzin, A.; Messina, A.; Meyer, J.; Milic, A.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Negri, G.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Rodrigues, L.; Roe, S.; Ruiz-Martinez, A.; Salzburger, A.; Savu, D. O.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van der Ster, D.; van Eldik, N.; van Woerden, M. C.; Vandelli, W.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Boveia, A.; Cheng, Y.; Facini, G.; Fiascaris, M.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Li, H. L.; Meehan, S.; Melachrinos, C.; Merritt, F. S.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Shochet, M. J.; Tompkins, L.; Vukotic, I.; Webster, J. S.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carquin, E.; Diaz, M. A.; Vogel, M.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lu, F.; Ouyang, Q.; Ren, H.; Shan, L. Y.; Sun, X.; Wang, J.; Xu, D.; Yao, L.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guan, L.; Han, L.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, K.; Liu, Y.; Peng, H.; Song, H. Y.; Xu, L.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Anhui, Peoples R China. [Chen, S.; Li, Y.; Wang, C.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200030, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. 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[Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartmento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Palka, M.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hoffman, J.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Sekula, S. J.; Stroynowski, R.; Wang, H.; Ye, S.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Lou, X.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Camarda, S.; Dassoulas, J. A.; Deterre, C.; Dietrich, J.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Belenguer, M. Jimenez; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Medinnis, M.; Moenig, K.; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Hamburg, Germany. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Camarda, S.; Dassoulas, J. A.; Deterre, C.; Dietrich, J.; Filipuzzi, M.; Glazov, A.; Fajardo, L. S. Gomez; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Belenguer, M. Jimenez; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Medinnis, M.; Moenig, K.; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Kobel, M.; Mader, W. F.; Morgenstern, M.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Oh, S. H.; Pollard, C. S.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Prokofiev, K.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Buescher, D.; Coniavitis, E.; Consorti, V.; Dao, V.; Di Simone, A.; Fehling-Kaschek, M.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Madar, R.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Rave, T. C.; Ronzani, M.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; von Radziewski, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Alexandre, G.; Aloisio, A.; Ancu, L. S.; Barone, G.; Bell, P. J.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Bucci, F.; Toro, R. Camacho; Clark, A.; Delitzsch, C. M.; della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Nektarijevic, S.; Nessi, M.; Nikolics, K.; Picazio, A.; Pohl, M.; Rosbach, K.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Bates, R. L.; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; O'Shea, V.; Barrera, C. Oropeza; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; Saxon, D. H.; Smith, K. M.; St Denis, R. D.; Stewart, G. A.; Thompson, A. S.; Wright, M.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bierwagen, K.; Bindi, M.; Blumenschein, U.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Hensel, C.; Kareem, M. J.; Kawamura, G.; Keil, M.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Stolte, P.; Schroeder, T. Vazquez; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS, IN2P3, Lab Phys Subat & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Butler, B.; Catastini, P.; Conti, G.; Franklin, M.; Huth, J.; Ippolito, V.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Yen, A. L.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A.; Brandt, O.; Davygora, Y.; Dietzsch, T. A.; Dunford, M.; Hanke, P.; Hofmann, J. I.; Jongmanns, J.; Khomich, A.; Kluge, E. -E.; Laier, H.; Lang, V. S.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Franz, S.; Jussel, P.; Kneringer, E.; Lukas, W.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Mallik, U.; Mandrysch, R.; Morange, N.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Kazarinov, M. Y.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Topilin, N. D.; Vinogradov, V. 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T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, RA-1900 La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Allison, L. J.; Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, Lecce, Italy. [Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. 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A.; Cooper-Smith, N. J.; Cowan, G.; Duguid, L.; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Rose, M.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Cooper, B. D.; Davison, A. R.; Davison, P.; Falla, R. J.; Gregersen, K.; Gutschow, C.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Korn, A.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, M. I.; Pilkington, A. D.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Bernius, C.; Greenwood, Z. D.; Jana, D. K.; Sawyer, L.; Sircar, A.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Meirose, B.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Inst Fys, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Blum, W.; Buescher, V.; Caputo, R.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Goeringer, C.; Heck, T.; Hohlfeld, M.; Hsu, P. J.; Huelsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lin, T. H.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Meyer, C.; Moreno, D.; Moritz, S.; Mueller, T.; Poettgen, R.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Almond, J.; Borri, M.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Peters, R. F. Y.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Robinson, J. E. M.; Schwanenberger, C.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Bertella, C.; Chen, L.; Clemens, J. C.; Coadou, Y.; Diglio, S.; Djama, F.; Feligioni, L.; Gao, J.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Clemens, J. C.; Coadou, Y.; Diglio, S.; Djama, F.; Feligioni, L.; Gao, J.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Brau, B.; Colon, G.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Mantifel, R.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Jennens, D.; Kubota, T.; Limosani, A.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Urquijo, P.; Volpi, M.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Dubbert, J.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Harper, D.; Levin, D.; Liu, L.; Long, J. D.; Lu, N.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Panikashvili, N.; Qian, J.; Schwarz, T. A.; Searcy, J.; Thun, R. P.; Wilson, A.; Wu, Y.; Xu, L.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Bromberg, C.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Koll, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Citterio, M.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Perini, L.; Pizio, C.; Ragusa, F.; Simoniello, R.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Tikhomirov, V. O.; Timoshenko, S.; Vorobev, K.] Moscow Engn & Phys Inst MEPhI, Moscow, Russia. [Boldyrev, A. 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G.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Pahl, C.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Spettel, F.; Stern, S.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Hasegawa, M.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Patricelli, S.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Chiefari, G.; Di Donato, C.; Giordano, R.; Merola, L.; Patricelli, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Klok, P. F.; Konig, A. C.; Salvucci, A.; Struebig, A.] Radboud Univ Nijmegen, Nikhef, Inst Math Astrophys & Particle Phys, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, A.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Oussoren, K. P.; Pani, P.; Salek, D.; Valencic, N.; Van den Wollenberg, W.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Oussoren, K. P.; Pani, P.; Salek, D.; Valencic, N.; Van den Wollenberg, W.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.] Univ Amsterdam, Amsterdam, Netherlands. [Burghgrave, B.; Calkins, R.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Skovpen, K. Yu.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, New York, NY 10003 USA. [Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Tannenwald, B. B.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Bertsche, C.; Bertsche, D.; Gutierrez, P.; Hasib, A.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Bousson, N.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] CNRS, IN2P3, F-91405 Orsay, France. [Endo, M.; Hanagaki, K.; Lee, J. S. H.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Gjelsten, B. K.; Gramstad, E.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Read, A. L.; Rohne, O.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Apolle, R.; Barr, A. J.; Behr, K.; Boddy, C. R.; Buckingham, R. M.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; King, R. S. B.; Kogan, L. A.; Lewis, A.; Livermore, S. S. A.; Nickerson, R. B.; Pachal, K.; Pinder, A.; Ryder, N. C.; Sawyer, C.; Short, D.; Tseng, J. C-L.; Vickey, T.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Meyer, C.; Ospanov, R.; Saxon, J.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Vanguri, R.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchini, L.; Boudreau, J.; Cleland, W.; Escobar, C.; Kittelmann, T.; Mueller, J.; Prieur, D.; Sapp, K.; Su, J.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Anjos, N.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Do Valle Wemans, A.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Gonalo, R.; Jorge, P. M.; Lopes, L.; Machado Miguens, J.; Maio, A.; Maneira, J.; Marques, C. N.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Tavares Delgado, A.; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Machado Miguens, J.; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Tavares Delgado, A.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. [Do Valle Wemans, A.] Univ Nova Lisboa, Dept Fis, Caparica, Portugal. [Do Valle Wemans, A.] Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Bohm, J.; Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Gallus, P.; Gunther, J.; Jakubek, J.; Kohout, Z.; Kral, V.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolezal, Z.; Faltova, J.; Kodys, P.; Leitner, R.; Pleskot, V.; Reznicek, P.; Rybar, M.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] Inst High Energy Phys, State Res Ctr, Protvino, Russia. [Adye, T.; Apolle, R.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Benslama, K.] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Dionisi, C.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Sidoti, A.; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; Di Domenico, A.; Dionisi, C.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Iuppa, R.; Liberti, B.; Mazzaferro, L.; Paolozzi, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Iuppa, R.; Mazzaferro, L.; Paolozzi, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Stanescu, C.; Taccini, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Taccini, C.; Trovatelli, M.] Univ Rome Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.] Reseau Univ Phys Hautes Energies Univ Hassan II, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA, Fac Sci Semlalia, Marrakech, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [Cherkaoui El Moursli, R.; Fassi, F.; Haddad, N.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Grabas, H. M. X.; Guyot, C.; Hanna, R.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mal, P.; Mansoulie, B.; Martinez, H.; Meric, N.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.; Tsionou, D.; Vranjes, N.; Xiao, M.] CEA Saclay, Commiss Energie Atom & Energies Alternat, DSM IRFU, Inst Rech Lois Fondament Univers, F-91191 Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grillo, A. A.; Kuhl, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; De Bruin, P. H. Sales; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Paredes, B. Lopez; Miyagawa, P. S.; Paganis, E.; Suruliz, K.; Tovey, D. R.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Dawe, E.; O'Neil, D. C.; Stelzer, B.; Tanasijczuk, A. J.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Mayes, J. Backus; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Kocian, M.; Kogan, L. A.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nef, P. D.; Nelson, T. K.; Piacquadio, G.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Strauss, E.; Su, D.; Swiatlowski, M.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Federic, P.; Plazak, L.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Connell, S. H.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Carrillo-Montoya, G. D.; Chen, X.; Hamity, G. N.; Hsu, C.; Garcia, B. R. Mellado; Ruan, X.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.] Stockholm Univ, Dept Phys, Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Gellerstedt, K.; Hellman, S.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Sjolin, J.; Strandberg, S.; Tylmad, M.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Bartsch, V.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Chu, M. L.; Hou, S.; Jamin, D. O.; Lee, C. A.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Ren, Z. L.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, C.; Wang, S. M.; Weng, Z.; Zhang, L.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Guttman, N.; Munwes, Y.; Oren, Y.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kordas, K.; Kouskoura, V.; Leisos, A.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.; Sidiropoulou, O.] Aristotle Univ Thessaloniki, Dept Phys, Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, Y.; Nobe, T.; Pettersson, N. E.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Brelier, B.; Chau, C. C.; Ilic, N.; Keung, J.; Krieger, P.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Schramm, S.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Fortin, D.; Gingrich, D. M.; Koutsman, A.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Taffard, A.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Bustos, A. C. Florez; Ramos, J. A. Manjarres; Palacino, G.; Qureshi, A.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Rao, K.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Pinamonti, M.; Quayle, W. B.; Shaw, K.; Soualah, R.] Ist Nazl Fis Nucl, Sez Trieste, Grp Collegato Udine, Udine, Italy. [Acharya, B. S.; Quayle, W. B.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Alhroob, M.; Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Pinamonti, M.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Coggeshall, J.; Errede, D.; Errede, S.; Lie, K.; Liss, T. M.; Neubauer, M. S.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Brenner, R.; Buszello, C. P.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garca, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garca, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Rodrigues, L.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, G.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garca, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garca, C.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Ferrer, A.; Fiorini, L.; Garca, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] CSIC, Valencia, Spain. [Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Bansal, V.; Berghaus, F.; Bernlochner, F. U.; David, C.; Fincke-Keeler, M.; Hamano, K.; Hill, E.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Marino, C. P.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.; Venturi, M.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Beckingham, M.; Farrington, S. M.; Harrison, P. F.; Janus, M.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Kimura, N.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Barak, L.; Bressler, S.; Citron, Z. 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A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Mal, P.] Natl Inst Sci Educ & Res, Sch Phys Sci, Bhubaneswar, Orissa, India. [Messina, A.] Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Pinamonti, M.] Scuola Int Super Studi Avanzati, SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Shi, L.; Soh, D. A.; Weng, Z.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Toth, J.] Wigner Res Ctr Phys, Inst Nucl & Particle Phys, Budapest, Hungary. [Wildt, M. A.] Univ Hamburg, Inst Expt Phys, Hamburg, Germany. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur 59100, Malaysia. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France. RI Capua, Marcella/A-8549-2015; Tartarelli, Giuseppe Francesco/A-5629-2016; Fassi, Farida/F-3571-2016; la rotonda, laura/B-4028-2016; Fabbri, Laura/H-3442-2012; Gutierrez, Phillip/C-1161-2011; Gerbaudo, Davide/J-4536-2012; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Peleganchuk, Sergey/J-6722-2014; Yang, Haijun/O-1055-2015; Monzani, Simone/D-6328-2017; Li, Liang/O-1107-2015; Garcia, Jose /H-6339-2015; Korol, Aleksandr/A-6244-2014; Olshevskiy, Alexander/I-1580-2016; Snesarev, Andrey/H-5090-2013; Ventura, Andrea/A-9544-2015; Kantserov, Vadim/M-9761-2015; BESSON, NATHALIE/L-6250-2015; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; KHODINOV, ALEKSANDR/D-6269-2015; Staroba, Pavel/G-8850-2014; Gauzzi, Paolo/D-2615-2009; Mindur, Bartosz/A-2253-2017; Smirnova, Oxana/A-4401-2013; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Wemans, Andre/A-6738-2012; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; Perrino, Roberto/B-4633-2010; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Zhukov, Konstantin/M-6027-2015; Shmeleva, Alevtina/M-6199-2015; Gavrilenko, Igor/M-8260-2015; Tikhomirov, Vladimir/M-6194-2015; Chekulaev, Sergey/O-1145-2015; Warburton, Andreas/N-8028-2013; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; De, Kaushik/N-1953-2013; Carvalho, Joao/M-4060-2013; Mashinistov, Ruslan/M-8356-2015; Della Pietra, Massimo/J-5008-2012; Petrucci, Fabrizio/G-8348-2012; Negrini, Matteo/C-8906-2014; Ferrer, Antonio/H-2942-2015; Brooks, William/C-8636-2013; White, Ryan/E-2979-2015; Villa, Mauro/C-9883-2009; Grancagnolo, Sergio/J-3957-2015; Doyle, Anthony/C-5889-2009; spagnolo, stefania/A-6359-2012; Tassi, Enrico/K-3958-2015; Ciubancan, Liviu Mihai/L-2412-2015; Connell, Simon/F-2962-2015; Bosman, Martine/J-9917-2014; Livan, Michele/D-7531-2012; Joergensen, Morten/E-6847-2015; Boyko, Igor/J-3659-2013; Mitsou, Vasiliki/D-1967-2009; Di Domenico, Antonio/G-6301-2011; Carquin, Edson/G-5221-2015; Mir, Lluisa-Maria/G-7212-2015; Riu, Imma/L-7385-2014; Cabrera Urban, Susana/H-1376-2015; Costa, Maria Jose/H-5962-2015; Cavalli-Sforza, Matteo/H-7102-2015 OI Capua, Marcella/0000-0002-2443-6525; Di Micco, Biagio/0000-0002-4067-1592; Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; Fassi, Farida/0000-0002-6423-7213; la rotonda, laura/0000-0002-6780-5829; Osculati, Bianca Maria/0000-0002-7246-060X; Giorgi, Filippo Maria/0000-0003-1589-2163; Coccaro, Andrea/0000-0003-2368-4559; Castro, Nuno/0000-0001-8491-4376; Veneziano, Stefano/0000-0002-2598-2659; Price, Darren/0000-0003-2750-9977; Fabbri, Laura/0000-0002-4002-8353; Gerbaudo, Davide/0000-0002-4463-0878; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Monzani, Simone/0000-0002-0479-2207; Li, Liang/0000-0001-6411-6107; Korol, Aleksandr/0000-0001-8448-218X; Giordani, Mario/0000-0002-0792-6039; Olshevskiy, Alexander/0000-0002-8902-1793; Ventura, Andrea/0000-0002-3368-3413; Kantserov, Vadim/0000-0001-8255-416X; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Gauzzi, Paolo/0000-0003-4841-5822; Mindur, Bartosz/0000-0002-5511-2611; Smirnova, Oxana/0000-0003-2517-531X; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Wemans, Andre/0000-0002-9669-9500; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; Perrino, Roberto/0000-0002-5764-7337; SULIN, VLADIMIR/0000-0003-3943-2495; Vykydal, Zdenek/0000-0003-2329-0672; Tikhomirov, Vladimir/0000-0002-9634-0581; Warburton, Andreas/0000-0002-2298-7315; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; De, Kaushik/0000-0002-5647-4489; Carvalho, Joao/0000-0002-3015-7821; Mashinistov, Ruslan/0000-0001-7925-4676; Della Pietra, Massimo/0000-0003-4446-3368; Petrucci, Fabrizio/0000-0002-5278-2206; Negrini, Matteo/0000-0003-0101-6963; Ferrer, Antonio/0000-0003-0532-711X; Brooks, William/0000-0001-6161-3570; White, Ryan/0000-0003-3589-5900; Villa, Mauro/0000-0002-9181-8048; Grancagnolo, Sergio/0000-0001-8490-8304; Doyle, Anthony/0000-0001-6322-6195; spagnolo, stefania/0000-0001-7482-6348; Ciubancan, Liviu Mihai/0000-0003-1837-2841; Connell, Simon/0000-0001-6000-7245; Bosman, Martine/0000-0002-7290-643X; Livan, Michele/0000-0002-5877-0062; Joergensen, Morten/0000-0002-6790-9361; Boyko, Igor/0000-0002-3355-4662; Mitsou, Vasiliki/0000-0002-1533-8886; Di Domenico, Antonio/0000-0001-8078-2759; Carquin, Edson/0000-0002-7863-1166; Mir, Lluisa-Maria/0000-0002-4276-715X; Riu, Imma/0000-0002-3742-4582; FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union; ERC; NSRF; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; ISF, Israel; MINERVA, Israel; GIF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; NCN, Poland; GRICES, Portugal; FCT, Portugal; MNE/IFA, Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, of Bern and Geneva, Switzerland; SNSF of Bern and Geneva, Switzerland; Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC; Royal Society and Leverhulme Trust, United Kingdom; DOE; NSF, United States of America FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; ISF, MINERVA, GIF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 80 TC 85 Z9 85 U1 17 U2 69 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD MAR 9 PY 2015 VL 91 IS 5 AR 052007 DI 10.1103/PhysRevD.91.052007 PG 25 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CC8MR UT WOS:000350623300001 ER PT J AU Collins, L Jesse, S Balke, N Rodriguez, BJ Kalinin, S Li, Q AF Collins, Liam Jesse, Stephen Balke, Nina Rodriguez, Brian J. Kalinin, Sergei Li, Qian TI Band excitation Kelvin probe force microscopy utilizing photothermal excitation SO APPLIED PHYSICS LETTERS LA English DT Article ID LABEL-FREE; RESOLUTION; NANOSCALE; INTERFACE; CORROSION; DYNAMICS; ARTIFACT; DEVICES AB A multifrequency open loop Kelvin probe force microscopy (KPFM) approach utilizing photothermal as opposed to electrical excitation is developed. Photothermal band excitation (PthBE)-KPFM is implemented here in a grid mode on a model test sample comprising a metal-insulator junction with local charge-patterned regions. Unlike the previously described open loop BE-KPFM, which relies on capacitive actuation of the cantilever, photothermal actuation is shown to be highly sensitive to the electrostatic force gradient even at biases close to the contact potential difference (CPD). PthBE-KPFM is further shown to provide a more localized measurement of true CPD in comparison to the gold standard ambient KPFM approach, amplitude modulated KPFM. Finally, PthBE-KPFM data contain information relating to local dielectric properties and electronic dissipation between tip and sample unattainable using conventional single frequency KPFM approaches. (C) 2015 AIP Publishing LLC. C1 [Collins, Liam; Rodriguez, Brian J.] Univ Coll Dublin, Sch Phys, Dublin 4, Ireland. [Collins, Liam; Rodriguez, Brian J.] Univ Coll Dublin, Conway Inst Biomol & Biomed Res, Dublin 4, Ireland. [Jesse, Stephen; Balke, Nina; Kalinin, Sergei; Li, Qian] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Collins, L (reprint author), Univ Coll Dublin, Sch Phys, Dublin 4, Ireland. EM Liam.Collins@ucdconnect.ie RI Balke, Nina/Q-2505-2015; Collins, Liam/A-3833-2016; Jesse, Stephen/D-3975-2016; OI Balke, Nina/0000-0001-5865-5892; Collins, Liam/0000-0003-4946-9195; Jesse, Stephen/0000-0002-1168-8483; Kalinin, Sergei/0000-0001-5354-6152 FU Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. DOE FX This research was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. DOE. Personal support was provided by the U.S. DOE, Basic Energy Sciences, Materials Sciences and Engineering Division through the Office of Science Early Career Research Program (N.B. and Q.L.). NR 40 TC 4 Z9 4 U1 5 U2 28 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAR 9 PY 2015 VL 106 IS 10 AR 104102 DI 10.1063/1.4913910 PG 5 WC Physics, Applied SC Physics GA CD9DM UT WOS:000351397600072 ER PT J AU Ergen, O Gibb, A Vazquez-Mena, O Regan, WR Zettl, A AF Ergen, Onur Gibb, Ashley Vazquez-Mena, Oscar Regan, William Raymond Zettl, Alex TI Metal insulator semiconductor solar cell devices based on a Cu2O substrate utilizing h-BN as an insulating and passivating layer SO APPLIED PHYSICS LETTERS LA English DT Article ID CUPROUS-OXIDE; PHOTOVOLTAIC PROPERTIES; CYANIDE TREATMENT; THIN-FILMS; DEFECTS; DEPOSITION; REDUCTION; HYDROGEN; CUO AB We demonstrate cuprous oxide (Cu2O) based metal insulator semiconductor Schottky (MIS-Schottky) solar cells with efficiency exceeding 3%. A unique direct growth technique is employed in the fabrication, and hexagonal boron nitride (h-BN) serves simultaneously as a passivation and insulation layer on the active Cu2O layer. The devices are the most efficient of any Cu2O based MIS-Schottky solar cells reported to date. (C) 2015 AIP Publishing LLC. C1 [Ergen, Onur; Gibb, Ashley; Vazquez-Mena, Oscar; Regan, William Raymond; Zettl, Alex] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Ergen, Onur; Gibb, Ashley; Vazquez-Mena, Oscar; Regan, William Raymond; Zettl, Alex] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Ergen, Onur; Gibb, Ashley; Vazquez-Mena, Oscar; Zettl, Alex] Univ Calif Berkeley, Kavli Energy Nanosci Inst, Berkeley, CA 94720 USA. [Ergen, Onur; Gibb, Ashley; Vazquez-Mena, Oscar; Zettl, Alex] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Zettl, A (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM azettl@berkeley.edu RI Zettl, Alex/O-4925-2016; OI Zettl, Alex/0000-0001-6330-136X; Regan, William/0000-0003-0143-9827; Vazquez Mena, Oscar/0000-0002-9351-550X; Vazquez-Mena, Oscacr/0000-0001-9054-5183 FU Office of Energy Research, Materials Sciences and Engineering Division of the U.S. Department of Energy [DE-AC02-05CH11231]; National Science Foundation within the Center of Integrated Nanomechanical Systems [EEC-0832819]; Office of Naval Research (MURI) [N00014-09-1066] FX This research was supported in part by the Office of Energy Research, Materials Sciences and Engineering Division of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231, which provided for the design of the experiment and Raman spectroscopy characterization; the National Science Foundation within the Center of Integrated Nanomechanical Systems, under Grant No. EEC-0832819, which provided for photovoltaic response characterization; and by the Office of Naval Research (MURI) under Grant No. N00014-09-1066, which provided for graphene growth and device assembly. O.E. acknowledges the support of SoloPower Systems, Inc., through X-ray characterization and the support of Professor Paul Alivisatos's group through quantum efficiency measurements. NR 30 TC 3 Z9 3 U1 4 U2 43 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAR 9 PY 2015 VL 106 IS 10 AR 103904 DI 10.1063/1.4914181 PG 4 WC Physics, Applied SC Physics GA CD9DM UT WOS:000351397600070 ER PT J AU Ma, W Herbert, FW Senanayake, SD Yildiz, B AF Ma, Wen Herbert, F. William Senanayake, Sanjaya D. Yildiz, Bilge TI Non-equilibrium oxidation states of zirconium during early stages of metal oxidation SO APPLIED PHYSICS LETTERS LA English DT Article ID X-RAY; THERMODYNAMIC STABILITY; PHOTOELECTRON-SPECTRA; QUANTITATIVE-ANALYSIS; THERMAL-OXIDATION; SURFACE OXIDATION; ROOM-TEMPERATURE; OXIDE-FILMS; ZR ALLOYS; OXYGEN AB The chemical state of Zr during the initial, self-limiting stage of oxidation on single crystal zirconium (0001), with oxide thickness on the order of 1 nm, was probed by synchrotron x-ray photoelectron spectroscopy. Quantitative analysis of the Zr 3d spectrum by the spectrum reconstruction method demonstrated the formation of Zr1+, Zr2+, and Zr3+ as non-equilibrium oxidation states, in addition to Zr4+ in the stoichiometric ZrO2. This finding resolves the long-debated question of whether it is possible to form any valence states between Zr-0 and Zr4+ at the metal-oxide interface. The presence of local strong electric fields and the minimization of interfacial energy are assessed and demonstrated as mechanisms that can drive the formation of these non-equilibrium valence states of Zr. (C) 2015 AIP Publishing LLC. C1 [Ma, Wen; Herbert, F. William; Yildiz, Bilge] MIT, Dept Nucl Sci & Engn, Lab Electrochem Interfaces, Cambridge, MA 02139 USA. [Herbert, F. William] MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA. [Senanayake, Sanjaya D.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. RP Yildiz, B (reprint author), MIT, Dept Nucl Sci & Engn, Lab Electrochem Interfaces, 77 Massachusetts Ave, Cambridge, MA 02139 USA. EM byildiz@mit.edu RI Senanayake, Sanjaya/D-4769-2009 OI Senanayake, Sanjaya/0000-0003-3991-4232 FU Laboratory Directed Research and Development program (LDRD) from Idaho National Laboratory [12026]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX We gratefully acknowledge the Laboratory Directed Research and Development program (LDRD Project No. 12026) from Idaho National Laboratory for financial support. The XPS measurements in this work were performed at the National Synchrotron Light Source, a DOE Office of Science User Facility and Brookhaven National Laboratory, supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Contract No. DE-AC02-98CH10886. We thank M. Youssef for useful discussions on the irreducibility of and point defects in ZrO2. We thank D. Mullins and P. Albercht at Oak Ridge National Laboratory for the use of the U12a beamline (Brookhaven National Laboratory) for XPS measurements. We thank J. Anibal Boscoboinik at Brookhaven National Laboratory for help with XPS measurements, and Kurt Broderick at Microsystems Technology Laboratories at MIT for help with sample preparation. NR 53 TC 1 Z9 1 U1 2 U2 26 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAR 9 PY 2015 VL 106 IS 10 AR 101603 DI 10.1063/1.4914180 PG 5 WC Physics, Applied SC Physics GA CD9DM UT WOS:000351397600014 ER PT J AU Shi, TT Yin, WJ Hong, F Zhu, K Yan, YF AF Shi, Tingting Yin, Wan-Jian Hong, Feng Zhu, Kai Yan, Yanfa TI Unipolar self-doping behavior in perovskite CH3NH3PbBr3 SO APPLIED PHYSICS LETTERS LA English DT Article ID ORGANOMETAL HALIDE PEROVSKITES; LEAD BROMIDE PEROVSKITE; SOLAR-CELL APPLICATIONS; AUGMENTED-WAVE METHOD; EFFICIENT; TRANSPORT; SEMICONDUCTORS; PERFORMANCE; DEPOSITION; ORIGINS AB Recent theoretical and experimental reports have shown that the perovskite CH3NH3PbI3 exhibits unique ambipolar self-doping properties. Here, we show by density-functional theory calculation that its sister perovskite, CH3NH3PbBr3, exhibits a unipolar self-doping behavior-CH3NH3PbBr3 presents only good p-type conductivity under thermal equilibrium growth conditions. We further show that despite a large bandgap of 2.2 eV, all dominant defects in CH3NH3PbBr3 create shallow levels, which partially explains the ultra-high open-circuit voltages achieved by CH3NH3PbBr3-based thin-film solar cells. Our results suggest that the perovskite CH3NH3PbBr3 can be both an excellent solar cell absorber and a promising low-cost hole-transport material for lead halide perovskite solar cells. (C) 2015 AIP Publishing LLC. C1 [Shi, Tingting; Yin, Wan-Jian; Hong, Feng; Yan, Yanfa] Univ Toledo, Dept Phys & Astron, Toledo, OH 43606 USA. [Shi, Tingting; Yin, Wan-Jian; Hong, Feng; Yan, Yanfa] Univ Toledo, Ctr Photovolta Innovat & Commercializat, Toledo, OH 43606 USA. [Zhu, Kai] Natl Renewable Energy Lab, Chem & Mat Sci Ctr, Golden, CO 80401 USA. RP Yan, YF (reprint author), Univ Toledo, Dept Phys & Astron, Toledo, OH 43606 USA. EM yanfa.yan@utoledo.edu RI Yin, Wanjian/F-6738-2013 FU U.S. Department of Energy (DOE) SunShot Initiative under the Next Generation Photovoltaics 3 program [DE-FOA-0000990]; Ohio Research Scholar Program; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; U.S. Department of Energy [DE-AC36-08-GO28308] FX This work was supported by the U.S. Department of Energy (DOE) SunShot Initiative under the Next Generation Photovoltaics 3 program (DE-FOA-0000990) and Ohio Research Scholar Program. This research used the resources of the Ohio Supercomputer Center and the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The work at the National Renewable Energy Laboratory is supported by the U.S. Department of Energy under Contract No. DE-AC36-08-GO28308. NR 41 TC 24 Z9 24 U1 15 U2 99 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAR 9 PY 2015 VL 106 IS 10 AR 103902 DI 10.1063/1.4914544 PG 5 WC Physics, Applied SC Physics GA CD9DM UT WOS:000351397600068 ER PT J AU Wang, Z Luk, TS Tan, YX Ji, DX Zhou, M Gan, QQ Yu, ZF AF Wang, Zhu Luk, Ting Shan Tan, Yixuan Ji, Dengxin Zhou, Ming Gan, Qiaoqiang Yu, Zongfu TI Tunneling-enabled spectrally selective thermal emitter based on flat metallic films SO APPLIED PHYSICS LETTERS LA English DT Article ID PHOTONIC CRYSTALS; LIGHT-ABSORPTION; BROAD-BAND; EMISSION; ABSORBER; REGION AB Infrared thermal emission from metals has important energy applications in thermophotovoltaics, radiative cooling, and lighting. Unfortunately, the emissivity of flat metal films is close to zero because the screening effect prevents metals' fluctuating currents from emitting to the far field. As a result, metal films are often used as reflecting mirrors instead of thermal emitters. Recently, nanostructured metals, such as metamaterials, have emerged as an interesting way to enhance and to spectrally control thermal emission based on plasmonic resonant effects. However, they require sophisticated lithography. Here, we proposed and experimentally demonstrated a completely different mechanism to achieve spectrally selective metallic emitters based on a tunneling effect. This effect allows a simple flat metal film to achieve a near-unity emissivity with controlled spectral selectivity for efficient heat-to-light energy conversion. (C) 2015 AIP Publishing LLC. C1 [Wang, Zhu; Tan, Yixuan; Zhou, Ming; Yu, Zongfu] Univ Wisconsin, Dept Elect & Comp Engn, Madison, WI 53706 USA. [Luk, Ting Shan] Sandia Natl Labs, Ctr Integrated Nanotechnol CINT, Albuquerque, NM 87185 USA. [Ji, Dengxin; Gan, Qiaoqiang] SUNY Buffalo, Dept Elect & Comp Engn, Buffalo, NY 14260 USA. RP Luk, TS (reprint author), Sandia Natl Labs, Ctr Integrated Nanotechnol CINT, POB 5800, Albuquerque, NM 87185 USA. EM tsluk@sandia.gov; zyu54@wisc.edu FU National Science Foundation [ECCS-1405201, ECCS-1425648]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04 94AL85000] FX The authors acknowledge the initial experimental help from Dr. Iltai Kim. The work was partially supported by National Science Foundation (Nos. ECCS-1405201 and ECCS-1425648). This work was performed, in part, at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04 94AL85000. NR 29 TC 8 Z9 8 U1 1 U2 44 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAR 9 PY 2015 VL 106 IS 10 AR 101104 DI 10.1063/1.4914886 PG 5 WC Physics, Applied SC Physics GA CD9DM UT WOS:000351397600004 ER PT J AU Ye, Z Zhang, F Sun, Y Mendelev, MI Ott, RT Park, E Besser, MF Kramer, MJ Ding, Z Wang, CZ Ho, KM AF Ye, Z. Zhang, F. Sun, Y. Mendelev, M. I. Ott, R. T. Park, E. Besser, M. F. Kramer, M. J. Ding, Z. Wang, C. -Z. Ho, K. -M. TI Discovery of a metastable Al20Sm4 phase SO APPLIED PHYSICS LETTERS LA English DT Article ID NANOCRYSTALLINE ALLOYS; GENETIC ALGORITHM; AMORPHOUS-ALLOYS; NANOQUASICRYSTALLINE; CRYSTALLIZATION; ALUMINUM AB We present an efficient genetic algorithm, integrated with experimental diffraction data, to solve a nanoscale metastable Al20Sm4 phase that evolves during crystallization of an amorphous magnetron sputtered Al90Sm10 alloy. The excellent match between calculated and experimental X-ray diffraction patterns confirms an accurate description of this metastable phase. Molecular dynamic simulations of crystal growth from the liquid phase predict the formation of disordered defects in the devitrified crystal. (C) 2015 AIP Publishing LLC. C1 [Ye, Z.; Zhang, F.; Sun, Y.; Mendelev, M. I.; Ott, R. T.; Park, E.; Besser, M. F.; Kramer, M. J.; Wang, C. -Z.; Ho, K. -M.] US DOE, Ames Lab, Ames, IA 50011 USA. [Sun, Y.; Ding, Z.; Ho, K. -M.] Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Anhui, Peoples R China. [Sun, Y.; Ding, Z.; Ho, K. -M.] Univ Sci & Technol China, Dept Phys, Hefei 230026, Anhui, Peoples R China. [Ho, K. -M.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. RP Ye, Z (reprint author), US DOE, Ames Lab, Ames, IA 50011 USA. EM zye@iastate.edu; kmh@ameslab.gov OI Park, Eun Soo/0000-0003-4185-6596; Sun, Yang/0000-0002-4344-2920 FU U.S. Department of Energy, Basic Energy Sciences, Division of Materials Science and Engineering [DE-AC02-07CH11358]; Advanced Photon Source, Argonne National Laboratory [DE-AC02-06CH11357] FX We would like to thank Jon Almer for his assistance in the HEXRD experiments. Work at Ames Laboratory was supported by the U.S. Department of Energy, Basic Energy Sciences, Division of Materials Science and Engineering, under Contract No. DE-AC02-07CH11358, including a grant of computer time at the National Energy Research Supercomputing Center (NERSC) in Berkeley, CA. The high-energy X-ray experiments were performed at the XOR beamline (sector 1) of the Advanced Photon Source, Argonne National Laboratory, under Grant No. DE-AC02-06CH11357. NR 17 TC 2 Z9 2 U1 4 U2 20 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAR 9 PY 2015 VL 106 IS 10 AR 101903 DI 10.1063/1.4914399 PG 4 WC Physics, Applied SC Physics GA CD9DM UT WOS:000351397600018 ER PT J AU Zhu, CH Harder, R Diaz, A Komanicky, V Barbour, A Xu, RQ Huang, XJ Liu, YH Pierce, MS Menzel, A You, H AF Zhu, Chenhui Harder, Ross Diaz, Ana Komanicky, Vladimir Barbour, Andi Xu, Ruqing Huang, Xiaojing Liu, Yaohua Pierce, Michael S. Menzel, Andreas You, Hoydoo TI Ptychographic x-ray imaging of surfaces on crystal truncation rod SO APPLIED PHYSICS LETTERS LA English DT Article ID COMPUTED-TOMOGRAPHY; MICROSCOPY; SCATTERING; RESOLUTION; REFLECTION; NANOSCALE AB Ptychography is a high-resolution imaging technique, which does not require lenses for image magnification and which provides phase contrast with high sensitivity. Here, we propose to use x-ray ptychography for the imaging of surface structure in crystalline samples. We show that ptychography can be used to image atomic step structures using coherent diffraction patterns recorded along the crystal truncation rod of a crystal surface. In a proof-of-concept experiment on a Pt (111) sample, we present ptychographic reconstructions showing features consistent with surface steps. Due to the penetration power of x-rays, this method could find interesting applications for the study of surface structures under buried interfaces or in harsh environments. (C) 2015 AIP Publishing LLC. C1 [Zhu, Chenhui; Barbour, Andi; Liu, Yaohua; You, Hoydoo] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Harder, Ross; Xu, Ruqing] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Diaz, Ana; Menzel, Andreas] Paul Scherrer Inst, CH-5232 Villigen, Switzerland. [Komanicky, Vladimir] Safarik Univ, Fac Sci, Kosice 04154, Slovakia. [Huang, Xiaojing] Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA. [Pierce, Michael S.] Rochester Inst Technol, Sch Phys & Astron, Rochester, NY 14623 USA. RP Zhu, CH (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM hyou@anl.gov RI Liu, Yaohua/B-2529-2009; Xu, Ruqing/K-3586-2012; You, Hoydoo/A-6201-2011; Diaz, Ana/I-4139-2013; Menzel, Andreas/C-4388-2012; Huang, Xiaojing/K-3075-2012; Pierce, Michael/D-5570-2014 OI Liu, Yaohua/0000-0002-5867-5065; Xu, Ruqing/0000-0003-1037-0059; You, Hoydoo/0000-0003-2996-9483; Diaz, Ana/0000-0003-0479-4752; Menzel, Andreas/0000-0002-0489-609X; Huang, Xiaojing/0000-0001-6034-5893; Pierce, Michael/0000-0002-9209-8556 FU Materials Sciences and Engineering Division; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-06CH11357]; Slovak Grant [VEGA 1/0782/12]; ERDF EU [ITMS 26220120005] FX We thank Jon Hiller for assistance in Electron Microscopy Center and Joan Vila-Comamala for providing the test pattern. The work at Materials Science Division (C.Z., A.B., Y.L., and H.Y.) was supported by the Materials Sciences and Engineering Division and the work at the Advanced Photon Source (R.H., R.X., and X.H.) and the Electron Microscopy Center by the Scientific User Facilities Division, of the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. The work was also in part performed at Swiss Light Source (A.D. and A.M.) and Rochester Institute of Technology (M.S.P.), and Safarik University (V.K.). The work at Safarik University was supported by Slovak Grant VEGA 1/0782/12 and ERDF EU Grant under Contract No. ITMS 26220120005. NR 31 TC 1 Z9 1 U1 4 U2 39 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAR 9 PY 2015 VL 106 IS 10 AR 101604 DI 10.1063/1.4914927 PG 5 WC Physics, Applied SC Physics GA CD9DM UT WOS:000351397600015 ER PT J AU Pena, J Bargar, JR Sposito, G AF Pena, Jasquelin Bargar, John R. Sposito, Garrison TI Copper sorption by the edge surfaces of synthetic birnessite nanoparticles SO CHEMICAL GEOLOGY LA English DT Article DE Manganese oxide; Birnessite; Trace metals; Copper; Sorption; EXAFS spectroscopy ID RAY-ABSORPTION SPECTROSCOPY; BIOGENIC MN OXIDES; MANGANESE OXIDES; PSEUDOMONAS-PUTIDA; CRYSTAL-STRUCTURE; HUMIC SUBSTANCES; OXIDATION-STATE; MODEL COMPOUNDS; HYDROUS OXIDES; NI AB We investigated the sorption of Cu by delta-MnO2, an analog for natural birnessite (layer-typeMnoxide) that is characterized by randomly stacked and curled nanosheets, a low to moderate vacancy content, and variable amounts of layer and interlayer Mn3+. The synthetic delta-MnO2 used in this study had a Na: Mn molar ratio of 0.13, an average manganese oxidation number (AMON) of 3.85 after reaction, a specific surface area of 254 m(2) g(-1) and a particle size of 2-4 nm in the ab plane. The maximum surface excess (q(max)) value at pH 6 estimated from sorption data of 0.72 (0.64-0.83, 95% confidence interval) mol Cu mol(-1) Mn far exceeded the nominal vacancy content for delta-MnO2 (ca. 6-11% mol vacancy mol(-1) Mn), thus implicating multiple binding sites for Cu. The large values of qmax and specific surface area of the mineral suggest a major role for surface sites at the particle edges relative to vacancy sites. The extended X-ray absorption fine structure (EXAFS) spectra from delta-MnO2 samples differ with respect to the EXAFS spectra for Cu(OH)(2), CuO, and Cu-3(CO3)(2)(OH)(2) and Cu-sorbed by biogenic MnO2. The Cu K-edge EXAFS spectra show two second-shell peaks that can be modeled with Mn and Cu near-neighbors. Copper appears to bind dominantly at particle edges of d-MnO2 as dimers or polynuclear surface species. This sorption mechanism is consistent with the moderate vacancy content of delta-MnO2 and explains the similarity in the EXAFS spectra from samples having surface loadings of 0.01 to 0.26 mol Cu mol(-1) Mn. The strong proclivity of Cu to bind on the edge surfaces of nanoparticulate birnessite leads to very large surface excesses of Cu without the formation of a discreet precipitate, making the surface sites at the particle edges the dominant sorption site for Cu. (C) 2015 Elsevier B.V. All rights reserved. C1 [Pena, Jasquelin] Univ Lausanne, Inst Earth Surface Dynam, CH-1015 Lausanne, Switzerland. [Bargar, John R.] SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource Directora, Stanford, CA 94025 USA. [Sposito, Garrison] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Dept Geochem, Berkeley, CA 94720 USA. RP Pena, J (reprint author), Univ Lausanne, Inst Earth Surface Dynam, CH-1015 Lausanne, Switzerland. EM jasquelin.pena@unil.ch; bargar@slac.stanford.edu; gsposito@berkeley.edu FU Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231]; Sandoz Family Foundation FX This research was supported by the Office of Basic Energy Sciences of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. HR-TEM images were acquired at the National Center for Electron Microscopy at Lawrence Berkeley National Laboratory. J. Pena acknowledges support from the Sandoz Family Foundation. Portions of this research were carried out at the Stanford Synchrotron Radiation Lightsource, a national user facility operated by Stanford University on behalf of the U.S. Department of Energy, Office of Basic Energy Sciences. NR 69 TC 10 Z9 10 U1 6 U2 36 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2541 EI 1878-5999 J9 CHEM GEOL JI Chem. Geol. PD MAR 9 PY 2015 VL 396 BP 196 EP 207 DI 10.1016/j.chemgeo.2014.12.021 PG 12 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA CE2TD UT WOS:000351670200017 ER PT J AU Zhang, S Yang, L DePaolo, DJ Steefel, CI AF Zhang, Shuo Yang, Li DePaolo, Donald J. Steefel, Carl I. TI Chemical affinity and pH effects on chlorite dissolution kinetics under geological CO2 sequestration related conditions SO CHEMICAL GEOLOGY LA English DT Article DE Chlorite dissolution kinetics; Chemical affinity effects; CO2 sequestration ID REACTIVE SURFACE-AREA; THERMODYNAMIC PROPERTIES; FREE-ENERGY; 80-DEGREES-C; RATES; 25-DEGREES-C; DEPENDENCE; TRANSPORT; MINERALS; GIBBSITE AB The kinetic dissolution of Flagstaff Hill chlorite (CCa-2 from Clay Minerals Society), (Mg4.55Al1.23Fe0.12) (Al1.04Si2.96)O-10(OH)(8), was investigated using a well-mixed flow-through reactor at 100 degrees C, pH values ranging from 3.0 to 7.5, and variable saturation states. The objective was to measure the dependence of chlorite dissolution rate on pH as well as on degree of undersaturation under conditions applicable to geologic carbon storage. A batch experiment was conducted to determine the equilibrium constant of the dissolution reaction at 100 degrees C for the chlorite mineral phase used in this study. A series of experiments was run at varying CO2 partial pressures (0-60 bars) and different flow rates (0.01-0.25 ml/min). We use our experimental results in conjunction with previously published data to separate the effects of pH and solution saturation state. At constant pH, the chlorite dissolution rate decreases slowly as a function of the Gibbs free energy of reaction (Delta G(r)), which is a quantitative measure of the degree of undersaturation. The undersaturation required (Delta G(r) > 100 kJ/mol) to reach a limiting far-from-equilibriumrate (the "dissolution plateau") is roughly an order of magnitude larger than expected from transition state theory, but similar to that determined for smectite (-Delta G(r) > 130 kJ/mol) (Cama et al., 2000). Hence, chlorite dissolution behaves as if the chlorite were close to equilibriumeven in solutions that are strongly undersaturated. The chlorite dissolution rate (R) as a function of pH and chemical affinity (Delta G(r)) at 100 degrees C can be fit reasonably well with the following expression: R = (10(-7.64)a(H)(1.05) + 10(-11.56)) {1-exp[-0.01677(vertical bar Delta G(r)vertical bar/RT)(1.3)]} The rate law obtained in this study provides a basis for modeling chlorite mineral dissolution over a range of pH and saturation conditions, which is essential in applications such as subsurface CO2 sequestration. (C) 2015 Elsevier B.V. All rights reserved. C1 [Zhang, Shuo; DePaolo, Donald J.] Univ Calif Berkeley, Earth & Planetary Sci, Berkeley, CA 94720 USA. [Zhang, Shuo; Yang, Li; DePaolo, Donald J.; Steefel, Carl I.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Zhang, S (reprint author), 16300 Pk Row Dr, Houston, TX 77084 USA. EM shuozhang@berkeley.edu; lyang@lbl.gov; djdepaolo@lbl.gov; cisteefel@lbl.gov RI Steefel, Carl/B-7758-2010; YANG, LI/F-9392-2010; OI Zhang, Shuo/0000-0002-2170-4299 FU Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy as part of the Energy Frontier Research Center Nanoscale Controls on Geologic CO2 [DE-AC02-CH11231] FX The work was supported by the Director, Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy as part of the Energy Frontier Research Center Nanoscale Controls on Geologic CO2 under contract no. DE-AC02-CH11231. NR 35 TC 9 Z9 9 U1 3 U2 25 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2541 EI 1878-5999 J9 CHEM GEOL JI Chem. Geol. PD MAR 9 PY 2015 VL 396 BP 208 EP 217 DI 10.1016/j.chemgeo.2015.01.001 PG 10 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA CE2TD UT WOS:000351670200018 ER PT J AU Aad, G Abbott, B Abdallah, J Khalek, SA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Agatonovic-Jovin, T Aguilar-Saavedra, JA Agustoni, M Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Aesson, TPA Akimoto, G Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Allbrooke, BMM Allison, LJ Allport, PP Almond, J Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Anduaga, XS Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonaki, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Apolle, R Arabidze, G Aracena, I Arai, Y Araque, JP Arce, ATH Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Arnaez, O Arnal, V Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Asai, S Asbah, N Ashkenazi, A Aman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Auerbach, B Augsten, K Aurousseau, M Avolio, G Azuelos, G Azuma, Y Baak, MA Baas, A Bacci, C Bachacou, H Bachas, K Backes, M Backhaus, M Mayes, JB Badescu, E Bagiacchi, P Bagnaia, P Bai, Y Bain, T Baines, JT Baker, OK Balek, P Balli, F Banas, E Banerjee, S Bannoura, AAE Bansal, V Bansil, HS Barak, L Baranov, SP Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, P Bartsch, V Bassalat, A Basye, A Bates, RL Batley, JR Battaglia, M Battistin, M Bauer, F Bawa, HS Beattie, MD Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, S Beckingham, M Becot, C Beddall, AJ Beddall, A Bedikian, S Bednyakov, VA Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, K Belanger-Champagne, C Bell, PJ Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Benslama, K Bentvelsen, S Berge, D Kuutmann, EB Berger, N Berghaus, F Beringer, J Bernard, C Bernat, P Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertoli, G Bertolucci, F Bertsche, C Bertsche, D Besana, MI Besjes, GJ Bylund, OB Bessner, M Besson, N Betancourt, C Bethke, S Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Bieniek, SP Bierwagen, K Biesiada, J Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Black, CW Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blazek, T Bloch, I Blocker, C Blum, W Blumenschein, U Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Bock, C Boddy, CR Boehler, M Boek, TT Bogaerts, JA Bogdanchikov, AG Bogouch, A Bohm, C Bohm, J Boisvert, V Bold, T Boldea, V Boldyrev, AS Bomben, M Bona, M Boonekamp, M Borisov, A Borissov, G Borri, M Borroni, S Bortfeldt, J Bortolotto, V Bos, K Boscherini, D Bosman, M Boterenbrood, H Boudreau, J Bouffard, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boutouil, S Boveia, A Boyd, J Boyko, IR Bracinik, J Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Brazzale, SF Brelier, B Brendlinger, K Brennan, AJ Brenner, R Bressler, S Bristow, K Bristow, TM Britton, D Brochu, FM Brock, I Brock, R Bromberg, C Bronner, J Brooijmans, G Brooks, T Brooks, WK Brosamer, J Brost, E Brown, J de Renstrom, PAB Bruncko, D Bruneliere, R Brunet, S Bruni, A Bruni, G Bruschi, M Bryngemark, L Buanes, T Buat, Q Bucci, F Buchholz, P Buckingham, RM Buckley, AG Buda, SI Budagov, IA Buehrer, F Bugge, L Bugge, MK Bulekov, O Bundock, AC Burckhart, H Burdin, S Burghgrave, B Burke, S Burmeister, I Busato, E Buscher, D Buscher, V Bussey, P Buszello, CP Butler, B Butler, JM Butt, AI Buttar, CM Butterworth, JM Butti, P Buttinger, W Buzatu, A Byszewski, M Urban, SC Caforio, D Cakir, O Calafiura, P Calandri, A Calderini, G Calfayan, P Calkins, R Caloba, LP Calvet, D Calvet, S Toro, RC Camarda, S Cameron, D Caminada, LM Armadans, RC Campana, S Campanelli, M Campoverde, A Canale, V Canepa, A Bret, MC Cantero, J Cantrill, R Cao, T Garrido, MDMC Caprini, I Caprini, M Capua, M Caputo, R Cardarelli, R Carli, T Carlino, G Carminati, L Caron, S Carquin, E Carrillo-Montoya, GD Carter, JR Carvalho, J Casadei, D Casado, MP Casolino, M Castaneda-Miranda, E Castelli, A Gimenez, VC Castro, NF Catastini, P Catinaccio, A Catmore, JR Cattai, A Cattani, G Caughron, S Cavaliere, V Cavalli, D Cavalli-Sforza, M Cavasinni, V Ceradini, 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CA ATLAS Collaboration TI Search for anomalous production of prompt same-sign lepton pairs and pair-produced doubly charged Higgs bosons with root s=8 TeV pp collisions using the ATLAS detector SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering; Beyond Standard Model; Particle and resonance production ID HEAVY MAJORANA NEUTRINOS; HADRON COLLIDERS; LHC; MASSES; VIOLATION; SIGNATURES; SYMMETRY; MODEL AB A low-background inclusive search for new physics in events with same-sign dileptons is presented. The search uses proton-proton collisions corresponding to 20.3 fb(-1) of integrated luminosity taken in 2012 at a centre-of-mass energy of 8TeV with the ATLAS detector at the LHC. Pairs of isolated leptons with the same electric charge and large transverse momenta of the type e(+/-) e(+/-), e(+/-) mu(+/-), and mu(+/-) mu(+/-) are selected and their invariant mass distribution is examined. No excess of events above the expected level of Standard Model background is found. The results are used to set upper limits on the cross-sections for processes beyond the Standard Model. Limits are placed as a function of the dilepton invariant mass within a fiducial region corresponding to the signal event selection criteria. Exclusion limits are also derived for a specific model of doubly charged Higgs boson production. C1 [Jackson, P.; Lee, L.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Edson, W.; Ernst, J.; Fischer, A.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Butt, A. I.; Czodrowski, P.; Gingrich, D. M.; Moore, R. W.; Pinfold, J. L.; Saddique, A.; Sbrizzi, A.; Vaque, F. Vives] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakir, O.; Ciftci, A. K.; Ciftci, R.; Yildiz, H. Duran; Kuday, S.] Ankara Univ, Dept Phys, TR-06100 Ankara, Turkey. [Yilmaz, M.] Gazi Univ, Dept Phys, Ankara, Turkey. 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Y.; Xu, L.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Li, Y.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200030, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Clermont Univ, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, CNRS, IN2P3, Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Chen, Y.; Cole, B.; Guo, J.; Hu, D.; Hughes, E. W.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Reale, V. Perez; Scherzer, M. I.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Wulf, E.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Simonyan, M.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Nazl Frascati Lab, Grp Collegato Cosenza, Arcavacata Di Rende, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dunford, M.; Dwuznik, M.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Palka, M.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hoffman, J.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Sekula, S. J.; Stroynowski, R.; Wang, H.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Lou, X.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Camarda, S.; Dassoulas, J. A.; Deterre, C.; Dietrich, J.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Belenguer, M. Jimenez; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Medinnis, M.; Moenig, K.; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Hamburg, Germany. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Camarda, S.; Dassoulas, J. A.; Deterre, C.; Dietrich, J.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Belenguer, M. Jimenez; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Medinnis, M.; Moenig, K.; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Zeuthen, Germany. [Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Wittig, T.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Kobel, M.; Leonhardt, K.; Mader, W. F.; Morgenstern, M.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Pollard, C. S.; Quadt, A.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, Sch Phys & Astron, SUPA, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Prokofiev, K.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Buescher, D.; Coniavitis, E.; Consorti, V.; Dao, V.; Di Simone, A.; Fehling-Kaschek, M.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Madar, R.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Rave, T. C.; Ronzani, M.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; von Radziewski, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Alexandre, G.; Ancu, L. S.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Bucci, F.; Toro, R. Camacho; Clark, A.; Delitzsch, C. M.; della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Nektarijevic, S.; Nikolics, K.; Picazio, A.; Pohl, M.; Rosbach, K.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartmento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys 4, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, GE-380086 Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, D-35390 Giessen, Germany. [Bates, R. L.; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; O'Shea, V.; Barrera, C. Oropeza; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; Saxon, D. H.; Smith, K. M.; Denis, R. D. St.; Stewart, G. A.; Thompson, A. S.; Wright, M.] Univ Glasgow, Sch Phys & Astron, SUPA, Glasgow, Lanark, Scotland. [Bierwagen, K.; Bindi, M.; Blumenschein, U.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Hensel, C.; Kawamura, G.; Keil, M.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Stolte, P.; Schroeder, T. Vazquez; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, D-37073 Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS, Lab Phys Subatom & Cosmol, IN2P3, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Butler, B.; Catastini, P.; Conti, G.; Franklin, M.; Huth, J.; Ippolito, V.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Yen, A. L.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A.; Brandt, O.; Davygora, Y.; Dietzsch, T. A.; Hanke, P.; Hofmann, J. I.; Jongmanns, J.; Khomich, A.; Kluge, E. -E.; Laier, H.; Lang, V. S.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Franz, S.; Jussel, P.; Kneringer, E.; Lukas, W.; Nagai, K.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Mallik, U.; Mandrysch, R.; Morange, N.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Kazarinov, M. Y.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Topilin, N. D.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Mitsui, S.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Inamaru, Y.; Kishimoto, T.; Kurashige, H.; Kurumida, R.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Verzini, M. J. Alconada; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, RA-1900 La Plata, Buenos Aires, Argentina. [Verzini, M. J. Alconada; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Allison, L. J.; Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Readioff, N. P.; Schnellbach, Y. J.; Sellers, G.; Vossebeld, J. H.; Waller, P.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bona, M.; Bret, M. Cano; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cooper-Smith, N. J.; Cowan, G.; Duguid, L.; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Rose, M.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Aloisio, A.; Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Cooper, B. D.; Davison, A. R.; Davison, P.; Falla, R. J.; Gregersen, K.; Gutschow, C.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Korn, A.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, M. I.; Pilkington, A. D.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Bernius, C.; Greenwood, Z. D.; Jana, D. K.; Sawyer, L.; Sircar, A.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Helgadottir, I. R.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Meirose, B.; Mjoernmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Inst Fys, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Blum, W.; Buescher, V.; Caputo, R.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Goeringer, C.; Heck, T.; Hohlfeld, M.; Hsu, P. J.; Huelsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Kopke, L.; Lin, T. H.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Meyer, C.; Moreno, D.; Moritz, S.; Mueller, T.; Poettgen, R.; Sander, H. G.; Schafer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, D-55122 Mainz, Germany. [Almond, J.; Borri, M.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Peters, R. F. Y.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Robinson, J. E. M.; Schwanenberger, C.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Bertella, C.; Clemens, J. C.; Coadou, Y.; Diglio, S.; Djama, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] Aix Marseille Univ, CNRS, CPPM, IN2P3, Marseille, France. [Bellomo, M.; Brau, B.; Colon, G.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Mantifel, R.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Jennens, D.; Kubota, T.; Limosani, A.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Urquijo, P.; Volpi, M.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Dubbert, J.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Harper, D.; Levin, D.; Li, L.; Long, J. D.; Lu, N.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Panikashvili, N.; Qian, J.; Searcy, J.; Thun, R. P.; Wilson, A.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Koll, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Citterio, M.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Perini, L.; Pizio, C.; Ragusa, F.; Simoniello, R.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] BI Stepanov Phys Inst, Natl Acad Sci Belarus, Minsk 220602, Byelarus. [Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] PN Lebedev Phys Inst, Acad Sci, Moscow 117924, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.; Vorobev, K.] Moscow Phys Engn Inst, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Becker, S.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Ebke, J.; Elmsheuser, J.; Heller, C.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Schieck, J.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Will, J. Z.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Manfredini, A.; Menke, S.; Moser, H. G.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Pahl, C.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Spettel, F.; Stern, S.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Patricelli, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Chiefari, G.; Di Donato, C.; Giordano, R.; Merola, L.; Patricelli, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartmento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Klok, P. F.; Konig, A. C.; Salvucci, A.; Struebig, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Oussoren, K. P.; Pani, P.; Salek, D.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Oussoren, K. P.; Pani, P.; Salek, D.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.] Univ Amsterdam, Amsterdam, Netherlands. [Burghgrave, B.; Calkins, R.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL USA. [Anisenkov, A. V.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Skovpen, K. Yu.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] Budker Inst Nucl Phys, SB RAS, Novosibirsk 630090, Russia. [Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, New York, NY 10003 USA. [Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Tannenwald, B. B.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Bertsche, C.; Bertsche, D.; Gutierrez, P.; Hasib, A.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Bousson, N.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. 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De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] CNRS, IN2P3, Orsay, France. [Endo, M.; Hanagaki, K.; Lee, J. S. H.; Nomachi, M.; Okamura, W.; Pitt, M.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Gjelsten, B. K.; Gramstad, E.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Read, A. L.; Rohne, O.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Apolle, R.; Barr, A. J.; Behr, K.; Boddy, C. R.; Buckingham, R. M.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; King, R. S. B.; Kogan, L. A.; Lewis, A.; Livermore, S. S. A.; Nickerson, R. B.; Pachal, K.; Pinder, A.; Ryder, N. C.; Sawyer, C.; Short, D.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Meyer, C.; Ospanov, R.; Saxon, J.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Vanguri, R.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Gunther, J.; Kittelmann, T.; Mueller, J.; Prieur, D.; Sapp, K.; Su, J.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Dos Santos, S. P. Amor; Amorim, A.; Anjos, N.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Wemans, A. Do Valle; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Miguens, J. Machado; Maio, A.; Maneira, J.; Marques, C. N.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] LIP, Lab Instrumentacao & Fis Expt Particulas, P-1000 Lisbon, Portugal. [Amorim, A.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, P-1699 Lisbon, Portugal. [Dos Santos, S. P. Amor; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Wemans, A. Do Valle] Univ Granada, CAFPE, Granada, Spain. [Wemans, A. Do Valle] Univ Nova Lisboa, Dept Fis, Caparica, Portugal. [Wemans, A. Do Valle] Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Bohm, J.; Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Gallus, P.; Jakubek, J.; Kohout, Z.; Kral, V.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Leitner, R.; Pleskot, V.; Reznicek, P.; Rybar, M.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] State Res Ctr Inst High Energy Phys, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Benslama, K.] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Bini, C.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Dionisi, C.; Gabrielli, A.; Lacava, F.; Luci, C.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Sidoti, A.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bini, C.; Di Domenico, A.; Dionisi, C.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Iuppa, R.; Liberti, B.; Mazzaferro, L.; Paolozzi, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Iuppa, R.; Mazzaferro, L.; Paolozzi, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Stanescu, C.; Taccini, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Taccini, C.; Trovatelli, M.] Univ Rome Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.] Univ Hassan 2, Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Techn Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA Marrakech, Marrakech, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Fassi, F.; Haddad, N.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Grabas, H. M. X.; Guyot, C.; Hanna, R.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mal, P.; Mansoulie, B.; Martinez, H.; Meric, N.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.; Tsionou, D.; Vranjes, N.; Xiao, M.] CEA Saclay, DSM IRFU, F-91191 Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grillo, A. A.; Kuhl, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; De Bruin, P. H. Sales; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Paredes, B. Lopez; Miyagawa, P. S.; Paganis, E.; Suruliz, K.; Tovey, D. R.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Burmeister, I.; Dawe, E.; Godfrey, J.; O'Neil, D. C.; Stelzer, B.; Tanasijczuk, A. J.; Torres, H.; Trottier-McDonald, M.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Mayes, J. Backus; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Kagan, M.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nef, P. D.; Nelson, T. K.; Piacquadio, G.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Strauss, E.; Su, D.; Swiatlowski, M.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Blazek, T.; Federic, P.; Plazak, L.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T. .] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Connell, S. H.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Carrillo-Montoya, G. D.; Chen, X.; Hamity, G. N.; Hsu, C.; Garcia, B. R. Mellado; Ruan, X.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Gellerstedt, K.; Hellman, S.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Sjolin, J.; Strandberg, S.; Tylmad, M.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Bee, C. P.; Campoverde, A.; Chen, K.; Engelmann, R.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Bartsch, V.; Cerri, A.; Barajas, C. A. Chavez; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Chu, M. L.; Hou, S.; Jamin, D. O.; Lee, C. A.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Ren, Z. L.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, C.; Wang, S. M.; Weng, Z.; Zhang, L.] Acad Sinica, Inst Phys, Taipei 115, Taiwan. [Abreu, H.; Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Guttman, N.; Munwes, Y.; Oren, Y.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kordas, K.; Kouskoura, V.; Leisos, A.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.; Sidiropoulou, O.] Aristotle Univ Thessaloniki, Dept Phys, Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Nobe, T.; Pettersson, N. E.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Brelier, B.; Chau, C. C.; Ilic, N.; Keung, J.; Krieger, P.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Schramm, S.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Canepa, A.; Chekulaev, S. V.; Fortin, D.; Koutsman, A.; Oram, C. J.; Codina, E. Perez; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Bustos, A. C. Florez; Ramos, J. A. Manjarres; Palacino, G.; Qureshi, A.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Quayle, W. B.; Shaw, K.; Soualah, R.] Ist Nazl Fis Nucl, Sez Trieste, Grp Collegato Udine, Udine, Italy. [Acharya, B. S.; De Sanctis, U.; Quayle, W. B.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Alhroob, M.; Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Pinamonti, M.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Coggeshall, J.; Errede, D.; Errede, S.; Lie, K.; Liss, T. M.; Neubauer, M. S.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Brenner, R.; Buszello, C. P.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.; Rao, K.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] IFIC, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Inst Microelect, IMB CNM, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Vos, M.] CSIC, Valencia, Spain. [Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC V5Z 1M9, Canada. [Albert, J.; Bansal, V.; Berghaus, F.; Bernlochner, F. U.; David, C.; Fincke-Keeler, M.; Hamano, K.; Hill, E.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Marino, C. P.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.; Venturi, M.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Beckingham, M.; Farrington, S. M.; Harrison, P. F.; Janus, M.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Kimura, N.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Barak, L.; Bressler, S.; Citron, Z. H.; Duchovni, E.; Gabizon, O.; Gross, E.; Groth-Jensen, J.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Milstein, D.; Pitt, M.; Roth, I.; Schaarschmidt, J.; Smakhtin, V.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Castillo, L. R. Flores; Hard, A. S.; Heng, Y.; Ji, H.; Ju, X.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Redelbach, A.; Schreyer, M.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Bannoura, A. A. E.; Barisonzi, M.; Becker, K.; Beermann, T. A.; Boek, T. T.; Braun, H. M.; Cornelissen, T.; Duda, D.; Ernis, G.; Fischer, J.; Fleischmann, S.; Flick, T.; Hamacher, K.; Harenberg, T.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Khoroshilov, A.; Kohlmann, S.; Lenzen, G.; Mattig, P.; Neumann, M.; Pataraia, S.; Sandhoff, M.; Sartisohn, G.; Wagner, W.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich C Phys, Wuppertal, Germany. [Adelman, J.; Baker, O. K.; Bedikian, S.; Cummings, J.; Czyczula, Z.; Demers, S.; Erdmann, J.; Garberson, F.; Golling, T.; Guest, D.; Henrichs, A.; Ideal, E.; Lagouri, T.; Leister, A. G.; Loginov, A.; Tipton, P.; Wall, R.; Walsh, B.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] Ctr Calcul Inst Natl Phys Nucl & Phys Particules, IN2P3, Villeurbanne, France. [Acharya, B. S.] Kings Coll London, Dept Phys, London, England. [Ahmadov, F.; Huseynov, N.; Javadov, N.] Azerbaijan Acad Sci, Inst Phys, Baku 370143, Azerbaijan. [Apolle, R.; Davies, E.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Azuelos, G.; Gingrich, D. M.; Oakham, F. G.; Savard, P.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Bawa, H. S.; Gao, Y. S.; Lowe, A. J.] Calif State Univ, Dept Phys, Fresno, CA USA. [Chelkov, G. A.] Tomsk State Univ, Tomsk 634050, Russia. 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[Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Shi, L.; Soh, D. A.; Weng, Z.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Tikhomirov, V. O.] Moscow Phys Engn Inst, Moscow, Russia. [Toth, J.] Inst Particle & Nucl Phys, Wigner Res Ctr Phys, Budapest, Hungary. [Vickey, T.] Univ Oxford, Dept Phys, Oxford, England. [Wang, C.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Wildt, M. A.] Univ Hamburg, Inst Expt Phys, Hamburg, Germany. [Xu, L.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur 59100, Malaysia. RP Aad, G (reprint author), Aix Marseille Univ, CNRS, CPPM, IN2P3, Marseille, France. 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Connell, Simon/F-2962-2015; Bosman, Martine/J-9917-2014; Boyko, Igor/J-3659-2013; Mitsou, Vasiliki/D-1967-2009; Fassi, Farida/F-3571-2016; la rotonda, laura/B-4028-2016; OI Gerbaudo, Davide/0000-0002-4463-0878; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Korol, Aleksandr/0000-0001-8448-218X; Giordani, Mario/0000-0002-0792-6039; Capua, Marcella/0000-0002-2443-6525; Di Micco, Biagio/0000-0002-4067-1592; Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; Ventura, Andrea/0000-0002-3368-3413; Kantserov, Vadim/0000-0001-8255-416X; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Goncalo, Ricardo/0000-0002-3826-3442; Gauzzi, Paolo/0000-0003-4841-5822; Mindur, Bartosz/0000-0002-5511-2611; Fabbri, Laura/0000-0002-4002-8353; 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Doyle, Anthony/0000-0001-6322-6195; spagnolo, stefania/0000-0001-7482-6348; Ferrando, James/0000-0002-1007-7816; Ciubancan, Liviu Mihai/0000-0003-1837-2841; Carquin, Edson/0000-0002-7863-1166; Mir, Lluisa-Maria/0000-0002-4276-715X; Livan, Michele/0000-0002-5877-0062; Brooks, William/0000-0001-6161-3570; Villa, Mauro/0000-0002-9181-8048; White, Ryan/0000-0003-3589-5900; Joergensen, Morten/0000-0002-6790-9361; Di Domenico, Antonio/0000-0001-8078-2759; Connell, Simon/0000-0001-6000-7245; Bosman, Martine/0000-0002-7290-643X; Boyko, Igor/0000-0002-3355-4662; Mitsou, Vasiliki/0000-0002-1533-8886; Fassi, Farida/0000-0002-6423-7213; la rotonda, laura/0000-0002-6780-5829; Osculati, Bianca Maria/0000-0002-7246-060X; Giorgi, Filippo Maria/0000-0003-1589-2163; Coccaro, Andrea/0000-0003-2368-4559; Della Volpe, Domenico/0000-0001-8530-7447; Castro, Nuno/0000-0001-8491-4376; Pina, Joao /0000-0001-8959-5044; Salamanna, Giuseppe/0000-0002-0861-0052; Veneziano, Stefano/0000-0002-2598-2659; Price, Darren/0000-0003-2750-9977 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET; ERC; NSRF; European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; ISF, Israel; MINERVA, Israel; GIF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; NCN, Poland; GRICES, Portugal; FCT, Portugal; MNE/IFA, Romania; MES of Russia; ROSATOM; Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZ. S, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Leverhulme Trust, United Kingdom; Royal Society, United Kingdom; DOE, United States of America; NSF, United States of America FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; ISF, MINERVA, GIF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW and NCN, Poland; GRICES and FCT, Portugal; MNE/IFA, Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZ. S, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFNCNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (U. K.) and BNL (U. S. A.) and in the Tier-2 facilities worldwide. NR 84 TC 23 Z9 23 U1 12 U2 82 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAR 9 PY 2015 IS 3 AR 041 DI 10.1007/JHEP03(2015)041 PG 48 WC Physics, Particles & Fields SC Physics GA CD7ZB UT WOS:000351313700001 ER PT J AU Aghasyan, M Avakian, H De Sanctis, E Gamberg, L Mirazita, M Musch, B Prokudin, A Rossi, P AF Aghasyan, M. Avakian, H. De Sanctis, E. Gamberg, L. Mirazita, M. Musch, B. Prokudin, A. Rossi, P. TI Studies of transverse momentum dependent parton distributions and Bessel weighting SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Deep Inelastic Scattering; Parton Model; QCD ID AZIMUTHAL DEPENDENCE; BOSON PRODUCTION; JEFFERSON LAB; LEPTOPRODUCTION; QUARK; MODEL; FRAGMENTATION; ASYMMETRIES; SCATTERING; COLLINS AB In this paper we present a new technique for analysis of transverse momentum dependent partondistribution functions, based on the Bessel weighting formalism. The procedure is applied to studies of the double longitudinal spin asymmetry in semi-inclusive deep inelastic scattering using a new dedicated Monte Carlo generator which includes quark intrinsic transverse momentum within the generalized parton model. Using a fully differential cross section for the process, the effect of four momentum conservation is analyzed using various input models for transverse momentum distributions and fragmentation functions. We observe a few percent systematic offset of the Bessel-weighted asymmetry obtained from Monte Carlo extraction compared to input model calculations, which is due to the limitations imposed by the energy and momentum conservation at the given energy/Q(2). We find that the Bessel weighting technique provides a powerful and reliable tool to study the Fourier transform of TMDs with controlled systematics due to experimental acceptances and resolutions with different TMD model inputs. C1 [Aghasyan, M.; De Sanctis, E.; Mirazita, M.; Rossi, P.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Aghasyan, M.] Inst Tecnol Aeronaut, DCTA, BR-12228900 Sao Jose Dos Campos, SP, Brazil. [Avakian, H.; Prokudin, A.; Rossi, P.] Jefferson Lab, Newport News, VA 23606 USA. [Gamberg, L.] Penn State Univ Berks, Dept Phys, Reading, PA 19610 USA. [Musch, B.] Univ Regensburg, Inst Theoret Phys, D-93040 Regensburg, Germany. RP Aghasyan, M (reprint author), Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. EM mher@jlab.org; avakian@jlab.org; Enzo.DeSanctis@lnf.infn.it; lpg10@psu.edu; marco.mirazita@lnf.infn.it; bmusch@ph.tum.de; prokudin@jlab.org; rossi@jlab.org FU U.S. Department of Energy [DE-AC05-06OR23177, DE-FG02-07ER41460]; CAPES [150324]; EU [283286]; Italian Istituto Nazionale di Fisica Nucleare FX This work is supported by the U.S. Department of Energy under Contract No. DE-AC05-06OR23177 (H.A., A.P., P.R.), No. DE-FG02-07ER41460 (L.G.), Science without borders young talent program from CAPES (contract number 150324 da CAPES), EU FP7 (HadronPhysics3, Grant Agreement number 283286) (M.A.), and the Italian Istituto Nazionale di Fisica Nucleare (M.A., H.A., E.De-S., M.M., P.R.). We thank M. Anselmino, D. Boer, S. Brodsky, U. D'Alesio, D. Hasch, A. Kotzinian, H. Matevosyan, and S. Melis for useful and stimulating discussions. We would like to thank the referee of this paper for his/her thoughtful comments that helped us to sharpen physics discussion and improve presentation of results. NR 80 TC 2 Z9 2 U1 0 U2 1 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAR 9 PY 2015 IS 3 AR 039 DI 10.1007/JHEP03(2015)039 PG 30 WC Physics, Particles & Fields SC Physics GA CD8SI UT WOS:000351365700001 ER PT J AU Park, S Koo, K Kim, K Ahn, H Lee, B Park, C Ryu, DY AF Park, Sungmin Koo, Kyosung Kim, Kyunginn Ahn, Hyungju Lee, Byeongdu Park, Cheolmin Ryu, Du Yeol TI Transition behavior of asymmetric polystyrene-b-poly(2-vinylpyridine) films: A stable hexagonally modulated layer structure SO POLYMER LA English DT Article DE Block copolymer; Thin film; Phase transition ID DIBLOCK COPOLYMER MELTS; BLOCK-COPOLYMER; THIN-FILMS; PERFORATED LAYER; DISORDER TRANSITION; PHASE-TRANSITIONS; GYROID PHASE; MORPHOLOGY; SUBSTRATE; POLYMERS AB The phase transitions in the films of an asymmetric polystyrene-b-poly(2-vinylpyridine) (PS-b-P2VP) were investigated by grazing incidence small-angle X-ray scattering (GISAXS) and transmission electron microscopy (TEM). Compared with the sequential transitions in the bulk, hexagonally perforated layer (HPL) -gyroid (GYR) - disorder (DIS) upon heating, the transitions in film geometry were dramatically changed with decreasing thickness due to the growing preferential interactions from substrate, resulting in a thickness-dependent transition diagram including four different morphologies of hexagonally modulated layer (HML), coexisting (HML and GYR), GYR, and DIS. Particularly in the films <= 10L(0), where L-0 is d-spacing at 150 degrees C, a stable HML structure was identified even above the order-to-disorder transition (ODT) temperature of the bulk, which was attributed to the suppressed compositional fluctuations by the enhanced substrate interactions. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Park, Sungmin; Koo, Kyosung; Kim, Kyunginn; Ryu, Du Yeol] Yonsei Univ, Dept Chem & Biomol Engn, Seoul 120749, South Korea. [Ahn, Hyungju] POSTECH, Dept Life Sci & Chem Mat, Pohang Accelerator Lab, Pohang 790834, South Korea. [Lee, Byeongdu] Argonne Natl Lab, Xray Sci Div, Adv Photon Source, Argonne, IL 60439 USA. [Park, Cheolmin] Yonsei Univ, Dept Mat Sci & Engn, Seoul 120749, South Korea. RP Ryu, DY (reprint author), Yonsei Univ, Dept Chem & Biomol Engn, 50 Yonsei Ro, Seoul 120749, South Korea. EM dyryu@yonsei.ac.kr RI Ryu, Du Yeol/G-8278-2012; OI Lee, Byeongdu/0000-0003-2514-8805 FU Samsung Research Funding Center of Samsung Electronics [SRFC-MA1301-03]; NRF - Ministry of Science, ICT & Future Planning (MSIP), Korea [2014R1A2A2A01004364] FX This research was supported by the Samsung Research Funding Center of Samsung Electronics under Project Number SRFC-MA1301-03 and NRF grants (2014R1A2A2A01004364) funded by the Ministry of Science, ICT & Future Planning (MSIP), Korea. NR 41 TC 4 Z9 4 U1 4 U2 43 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0032-3861 EI 1873-2291 J9 POLYMER JI Polymer PD MAR 9 PY 2015 VL 60 BP 32 EP 39 DI 10.1016/j.polymer.2015.01.022 PG 8 WC Polymer Science SC Polymer Science GA CD5GZ UT WOS:000351117300006 ER PT J AU Kurganov, AA Svec, F Kanateva, AY AF Kurganov, Alexander A. Svec, Frantisek Kanateva, Anastasiia Yu TI Flow induced conformational transitions of macromolecules and their effect on chromatographic separations SO POLYMER LA English DT Article DE Conformational transitions; Hydrodynamic chromatography; Size exclusion chromatography ID DILUTE POLYMER-SOLUTIONS; COIL-STRETCH TRANSITION; GEL-PERMEATION CHROMATOGRAPHY; BROWNIAN DYNAMICS SIMULATIONS; COLUMN HYDRODYNAMIC CHROMATOGRAPHY; SIZE-EXCLUSION CHROMATOGRAPHY; LIGHT-SCATTERING MEASUREMENTS; TRANSIENT ELONGATIONAL FLOW; NONPOROUS SILICA PARTICLES; OPEN MICROCAPILLARY TUBES AB The conformation of macromolecules is significantly affected, both in free flow as well as when flowing in a confined space. These effects play a major role when passing polymer molecules in solution through a porous system such as chromatographic column or membrane. Current theories take into account the conformational changes of polymer molecules caused by flow, and provide a description of the unusual behavior of macromolecules during chromatographic separation. Due to the changes in conformation, the flow can also cause degradation of polymers which have a very large molar mass. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Kurganov, Alexander A.; Kanateva, Anastasiia Yu] Russian Acad Sci, Topchiev Inst Petrochem Synth, Moscow 119991, Russia. [Svec, Frantisek] EO Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA USA. RP Kurganov, AA (reprint author), Russian Acad Sci, Topchiev Inst Petrochem Synth, Moscow 119991, Russia. EM kurganov@ips.ac.ru RI Foundry, Molecular/G-9968-2014 FU RFFI [13-03-00068]; Presidium of Russian Academy of Sciences [9]; Office of Science, Office of Basic Energy Sciences, Scientific User Facilities Division of the US Department of Energy [DE-AC02-05CH11231] FX We gratefully acknowledge support by RFFI Grant No. 13-03-00068 and by a Grant of Presidium of Russian Academy of Sciences (Program # 9). Work of FS on this project was performed at the Molecular Foundry, Lawrence Berkeley National Laboratory and supported by the Office of Science, Office of Basic Energy Sciences, Scientific User Facilities Division of the US Department of Energy, under Contract No. DE-AC02-05CH11231. NR 146 TC 2 Z9 2 U1 4 U2 15 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0032-3861 EI 1873-2291 J9 POLYMER JI Polymer PD MAR 9 PY 2015 VL 60 BP A1 EP A18 DI 10.1016/j.polymer.2015.01.010 PG 18 WC Polymer Science SC Polymer Science GA CD5GZ UT WOS:000351117300001 ER PT J AU Furukawa, H Muller, U Yaghi, OM AF Furukawa, Hiroyasu Mueller, Ulrich Yaghi, Omar M. TI "Heterogeneity within Order" in Metal-Organic Frameworks SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Review DE defects; heterogeneity; industrial chemistry; metal-organic frameworks; secondary building units ID ZEOLITIC IMIDAZOLATE FRAMEWORKS; POROUS COORDINATION POLYMERS; SECONDARY-BUILDING UNITS; CARBON-DIOXIDE; SURFACE-AREA; FUNCTIONAL-GROUPS; THIN-FILMS; INDUSTRIAL APPLICATIONS; CAPTURE PROPERTIES; SELECTIVE CAPTURE AB Metal-organic frameworks (MOFs) are constructed by linking inorganic units with organic linkers to make extended networks. Though more than 20000 MOF structures have been reported most of these are ordered and largely composed of a limited number of different kinds building units, and very few have multiple different building units (heterogeneous). Although heterogeneity and multiplicity is a fundamental characteristic of biological systems, very few synthetic materials incorporate heterogeneity without losing crystalline order. Thus, the question arises: how do we introduce heterogeneity into MOFs without losing their ordered structure? This Review outlines strategies for varying the building units within both the backbone of the MOF and its pores to produce the heterogeneity that is sought after. The impact this heterogeneity imparts on the properties of a MOF is highlighted. We also provide an update on the MOF industry as part of this themed issue for the 150th anniversary of BASF. C1 [Furukawa, Hiroyasu; Yaghi, Omar M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Chem, Div Mat Sci, Berkeley, CA 94720 USA. [Furukawa, Hiroyasu; Yaghi, Omar M.] Kavli Energy NanoSci Inst Berkeley, Berkeley, CA 94720 USA. [Furukawa, Hiroyasu; Yaghi, Omar M.] King Abdulaziz City Sci & Technol, Riyadh 11442, Saudi Arabia. [Mueller, Ulrich] BASF SE, Chem Res & Engn, D-67056 Ludwigshafen, Germany. RP Furukawa, H (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Chem, Div Mat Sci, Berkeley, CA 94720 USA. EM furukawa@berkeley.edu; ulrich.mueller@BASF.com; yaghi@berkeley.edu RI Furukawa, Hiroyasu/C-5910-2008; OI Furukawa, Hiroyasu/0000-0002-6082-1738; Yaghi, Omar/0000-0002-5611-3325 FU BASF SE (Ludwigshafen, Germany); U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Energy Frontier Research Center [DE-SC0001015]; U.S. Department of Defense, Defense Threat Reduction Agency [HDTRA 1-12-1-0053]; King Abdulaziz City of Science and Technology, Riyadh, Saudi Arabia FX We acknowledge Dr. Lena Arnold and Dr. Alex U. Czaja (BASF SE) for discussions of MOFs in industry, and Mr. K. E. Cordova and Dr. K. M. Choi (Yaghi group) for their valuable input. Financial support for MOF research in O.M.Y. laboratories is provided by BASF SE (Ludwigshafen, Germany); U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Energy Frontier Research Center grant DE-SC0001015; U.S. Department of Defense, Defense Threat Reduction Agency grant HDTRA 1-12-1-0053, and King Abdulaziz City of Science and Technology, Riyadh, Saudi Arabia. NR 121 TC 100 Z9 101 U1 66 U2 529 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD MAR 9 PY 2015 VL 54 IS 11 SI SI BP 3417 EP 3430 DI 10.1002/anie.201410252 PG 14 WC Chemistry, Multidisciplinary SC Chemistry GA CD0LZ UT WOS:000350766100019 PM 25586609 ER PT J AU Richards, G Gemmen, RS Williams, MC AF Richards, George Gemmen, Randall S. Williams, Mark C. TI Solid - state electrochemical heat engines SO INTERNATIONAL JOURNAL OF HYDROGEN ENERGY LA English DT Article DE Energy harvesting; Heat engine; Thermal charging; Electrolyser; Fuel cell ID CELL AB This paper explores the potential of using solid-state electrochemical heat engines (EHE) operating on reversible redox reactions to generate electric power using available thermal energy from natural and man-made sources. Electrochemical heat engines utilize and control the electrochemical potential of molecules undergoing redox reactions in a manner to produce electrical energy from thermal energy. The electrochemical potential of these redox pairs is a function of composition, temperature and pressure. EHE's in this paper exploit the change in basic thermodynamic properties with temperature. The EHE technology can be deployed using fuel cell and electrolyser combinations. It is quite interesting that for mature optimized EHE systems there is great potential for energy harvesting. Copyright (C) 2015, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved. C1 [Richards, George; Gemmen, Randall S.] Natl Energy Technol Lab, Morgantown, WV 26507 USA. [Williams, Mark C.] Natl Energy Technol Lab, URS, Morgantown, WV 26507 USA. RP Williams, MC (reprint author), Natl Energy Technol Lab, URS, 3610 Collins Ferry Rd, Morgantown, WV 26507 USA. EM george.richards@netl.doe.gov; randall.gemmen@netl.doe.gov; mark.willams@contr.netl.doe.gov FU US DOE NETL FX The authors would like to acknowledge the US DOE NETL for its support. NR 21 TC 1 Z9 1 U1 2 U2 6 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-3199 EI 1879-3487 J9 INT J HYDROGEN ENERG JI Int. J. Hydrog. Energy PD MAR 9 PY 2015 VL 40 IS 9 BP 3719 EP 3725 DI 10.1016/j.ijhydene.2015.01.043 PG 7 WC Chemistry, Physical; Electrochemistry; Energy & Fuels SC Chemistry; Electrochemistry; Energy & Fuels GA CD2PP UT WOS:000350921800013 ER PT J AU Yang, XL Hofmann, R Dapp, R van de Kamp, T Rolo, TD Xiao, XH Moosmann, J Kashef, J Stotzka, R AF Yang, Xiaoli Hofmann, Ralf Dapp, Robin van de Kamp, Thomas Rolo, Tomy dos Santos Xiao, Xianghui Moosmann, Julian Kashef, Jubin Stotzka, Rainer TI TV-based conjugate gradient method and discrete L-curve for few-view CT reconstruction of X-ray in vivo data SO OPTICS EXPRESS LA English DT Article ID TOTAL-VARIATION MINIMIZATION; DISTANCE PHASE RETRIEVAL; ILL-POSED PROBLEMS; IMAGE-RECONSTRUCTION; COMPUTED-TOMOGRAPHY; 1ST-ORDER METHOD; REGULARIZATION; PARAMETER; MICROTOMOGRAPHY; IMPLEMENTATION AB High-resolution, three-dimensional (3D) imaging of soft tissues requires the solution of two inverse problems: phase retrieval and the reconstruction of the 3D image from a tomographic stack of two-dimensional (2D) projections. The number of projections per stack should be small to accommodate fast tomography of rapid processes and to constrain X-ray radiation dose to optimal levels to either increase the duration of in vivo time-lapse series at a given goal for spatial resolution and/or the conservation of structure under X-ray irradiation. In pursuing the 3D reconstruction problem in the sense of compressive sampling theory, we propose to reduce the number of projections by applying an advanced algebraic technique subject to the minimisation of the total variation (TV) in the reconstructed slice. This problem is formulated in a Lagrangian multiplier fashion with the parameter value determined by appealing to a discrete L-curve in conjunction with a conjugate gradient method. The usefulness of this reconstruction modality is demonstrated for simulated and in vivo data, the latter acquired in parallel-beam imaging experiments using synchrotron radiation. (C) 2015 Optical Society of America C1 [Yang, Xiaoli; Dapp, Robin; Stotzka, Rainer] Karlsruhe Inst Technol, Inst Data Proc & Elect IPE, D-76344 Eggenstein Leopoldshafen, Germany. [Hofmann, Ralf; van de Kamp, Thomas; Rolo, Tomy dos Santos; Moosmann, Julian; Kashef, Jubin] Karlsruhe Inst Technol, Inst Photon Sci & Synchrotron Radiat IPS, D-76344 Eggenstein Leopoldshafen, Germany. [Xiao, Xianghui] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Yang, XL (reprint author), Karlsruhe Inst Technol, Inst Data Proc & Elect IPE, Hermann von Helmholtz Pl 1, D-76344 Eggenstein Leopoldshafen, Germany. EM xiaoli.yang@partner.kit.edu; ralf.hofmann2@kit.edu RI van de Kamp, Thomas/G-1440-2016; dos Santos Rolo, Tomy/F-5511-2016; Moosmann, Julian/D-7075-2013 OI van de Kamp, Thomas/0000-0001-7390-1318; dos Santos Rolo, Tomy/0000-0002-9771-3511; Moosmann, Julian/0000-0002-6761-7182 FU Helmholtz Portfolio Extension "Large Scale Data Management and Analysis"; Data Life Cycle Lab "Key Technologies"; U.S. DOE [DE-AC02-06CH11357]; Helmholtz Association of German Research Centers; China Scholarship Council (CSC); German Federal Ministry of Education and Research [05K12CK2, 05K12VH1]; European Commission [MP1207]; Deutsche Forschungsgemeinschaft; Karlsruhe Institute of Technology FX This work was supported by the Helmholtz Portfolio Extension "Large Scale Data Management and Analysis" and the Data Life Cycle Lab "Key Technologies". The data was acquired at ANKA's imaging beamline TOPO-TOMO and at beamline 32-ID of the Advanced Photon Source (APS). Use of APS was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. The authors would like to acknowledge generous support by both facilities and thank them for the provision of synchrotron radiation. R.H. would like to thank Madeleine Hertel and Steffen Hahn for performing quasiparticle phase retrieval on the frog data. X.Y. would like to thank the heads of IPE and IPS, Marc Weber and Tilo Baumbach, for their support and motivation to this paper. X.Y. would also like to acknowledge support by the Helmholtz Association of German Research Centers and the PhD scholarship from the China Scholarship Council (CSC). This research was partially funded by the German Federal Ministry of Education and Research under grant numbers 05K12CK2, 05K12VH1 and by COST action MP1207 supported by the European Commission. We acknowledge support by Deutsche Forschungsgemeinschaft and Open Access Publishing Fund of Karlsruhe Institute of Technology. NR 45 TC 5 Z9 6 U1 2 U2 24 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD MAR 9 PY 2015 VL 23 IS 5 BP 5368 EP 5387 DI 10.1364/OE.23.005368 PG 20 WC Optics SC Optics GA CD2BL UT WOS:000350878500002 PM 25836772 ER PT J AU Deng, JJ Nashed, YSG Chen, S Phillips, NW Peterka, T Ross, R Vogt, S Jacobsen, C Vine, DJ AF Deng, Junjing Nashed, Youssef S. G. Chen, Si Phillips, Nicholas W. Peterka, Tom Ross, Rob Vogt, Stefan Jacobsen, Chris Vine, David J. TI Continuous motion scan ptychography: characterization for increased speed in coherent x-ray imaging SO OPTICS EXPRESS LA English DT Article ID COMPUTED-TOMOGRAPHY; WAVE-FIELDS; DIFFRACTION; RESOLUTION; MICROSCOPY; RECONSTRUCTION; FLUORESCENCE; OPTICS AB Ptychography is a coherent diffraction imaging (CDI) method for extended objects in which diffraction patterns are acquired sequentially from overlapping coherent illumination spots. The object's complex transmission function can be reconstructed from those diffraction patterns at a spatial resolution limited only by the scattering strength of the object and the detector geometry. Most experiments to date have positioned the illumination spots on the sample using a move-settle-measure sequence in which the move and settle steps can take longer to complete than the measure step. We describe here the use of a continuous "fly-scan" mode for ptychographic data collection in which the sample is moved continuously, so that the experiment resembles one of integrating the diffraction patterns from multiple probe positions. This allows one to use multiple probe mode reconstruction methods to obtain an image of the object and also of the illumination function. We show in simulations, and in x-ray imaging experiments, some of the characteristics of fly-scan ptychography, including a factor of 25 reduction in the data acquisition time. This approach will become increasingly important as brighter x-ray sources are developed, such as diffraction limited storage rings. (C) 2015 Optical Society of America C1 [Deng, Junjing] Northwestern Univ, Appl Phys Program, Evanston, IL 60208 USA. [Nashed, Youssef S. G.; Peterka, Tom; Ross, Rob] Argonne Natl Lab, Math & Comp Sci Div, Argonne, IL 60439 USA. [Chen, Si; Vogt, Stefan; Jacobsen, Chris; Vine, David J.] Argonne Natl Lab, Xray Sci Div, Adv Photon Source, Argonne, IL 60439 USA. [Jacobsen, Chris] Northwestern Univ, Dept Phys & Astron, Evanston, IL 60208 USA. [Jacobsen, Chris] Northwestern Univ, Chem Life Proc Inst, Evanston, IL 60208 USA. [Phillips, Nicholas W.] La Trobe Univ, Ctr Excellence Adv Mol Imaging, Australian Res Council, Bundoora, Vic 3086, Australia. [Phillips, Nicholas W.] CSIRO Mfg Flagship, Parkville, Vic 3052, Australia. RP Jacobsen, C (reprint author), Argonne Natl Lab, Xray Sci Div, Adv Photon Source, Argonne, IL 60439 USA. EM cjacobsen@anl.gov RI Jacobsen, Chris/E-2827-2015; Vogt, Stefan/J-7937-2013; Vogt, Stefan/B-9547-2009 OI Jacobsen, Chris/0000-0001-8562-0353; Vogt, Stefan/0000-0002-8034-5513; Vogt, Stefan/0000-0002-8034-5513 FU NIH NIGMS [GM104530]; NIH/NCRR High End Instrumentation (HEI) grant as part of the American Recovery and Reinvestment Act (ARRA) [1S10RR029272-01]; U.S. DOE [DE-AC02-06CH11357] FX We thank R. Mak and Y. Sun for valuable discussions, K. Brister, C. Roehrig, J. VonOsinkski, and M. Bolbat for help during the experiments. We thank NIH NIGMS for support of this work under R01 grant GM104530. The Bionanoprobe is funded by NIH/NCRR High End Instrumentation (HEI) grant (1S10RR029272-01) as part of the American Recovery and Reinvestment Act (ARRA). Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. NR 36 TC 11 Z9 11 U1 3 U2 28 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD MAR 9 PY 2015 VL 23 IS 5 BP 5438 EP 5451 DI 10.1364/OE.23.005438 PG 14 WC Optics SC Optics GA CD2BL UT WOS:000350878500007 PM 25836777 ER PT J AU Burdet, N Shi, XW Parks, D Clark, JN Huang, XJ Kevan, SD Robinson, IK AF Burdet, Nicolas Shi, Xiaowen Parks, Daniel Clark, Jesse N. Huang, Xiaojing Kevan, Stephen D. Robinson, Ian K. TI Evaluation of partial coherence correction in X-ray ptychography SO OPTICS EXPRESS LA English DT Article ID QUANTITATIVE PHASE RETRIEVAL; ILLUMINATION AB Coherent X-ray Diffraction Imaging (CDI) and X-ray ptychography both heavily rely on the high degree of spatial coherence of the X-ray illumination for sufficient experimental data quality for reconstruction convergence. Nevertheless, the majority of the available synchrotron undulator sources have a limited degree of partial coherence, leading to reduced data quality and a lower speckle contrast in the coherent diffraction patterns. It is still an open question whether experimentalists should compromise the coherence properties of an X-ray source in exchange for a higher flux density at a sample, especially when some materials of scientific interest are relatively weak scatterers. A previous study has suggested that in CDI, the best strategy for the study of strong phase objects is to maintain a high degree of coherence of the illuminating X-rays because of the broadening of solution space resulting from the strong phase structures. In this article, we demonstrate the first systematic analysis of the effectiveness of partial coherence correction in ptychography as a function of the coherence properties, degree of complexity of illumination (degree of phase diversity of the probe) and sample phase complexity. We have also performed analysis of how well ptychographic algorithms refine X-ray probe and complex coherence functions when those variables are unknown at the start of reconstructions, for noise-free simulated data, in the case of both real-valued and highly-complex objects. (C) 2015 Optical Society of America C1 [Burdet, Nicolas; Robinson, Ian K.] UCL, London Ctr Nanotechnol, London WC1H 0AH, England. [Burdet, Nicolas; Robinson, Ian K.] Res Complex Harwell, Harwell OX11 0QF, Berks, England. [Shi, Xiaowen; Parks, Daniel; Kevan, Stephen D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Shi, Xiaowen; Parks, Daniel; Kevan, Stephen D.] Univ Oregon, Dept Phys, Eugene, OR 97401 USA. [Clark, Jesse N.] SLAC Natl Accelerator Lab, Stanford PULSE Inst, Menlo Pk, CA 94025 USA. [Clark, Jesse N.] DESY, Ctr Free Electron Laser Sci, D-22607 Hamburg, Germany. [Huang, Xiaojing] Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA. RP Shi, XW (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM xwshi@lbl.gov OI Kevan, Stephen/0000-0002-4621-9142 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Science and Engineering [DE-FG02 11ER46831]; Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02- 05CH11231]; UK Engineering and Physical Sciences Research Council (EPSRC) [EP/G068437/1, EP/I022562/1]; U.S. DOE [DE-AC02-06CH11357]; National Science Foundation [DMR-9724294]; Volkswagen Foundation FX The work of XS, DP, and SK was partially supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Science and Engineering under Grant No. DE-FG02 11ER46831. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02- 05CH11231.; The Research conducted at University College London, United Kingdom was carried out under grants EP/G068437/1 and EP/I022562/1 from the UK Engineering and Physical Sciences Research Council (EPSRC).; Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. Beamline 34-ID-C was built with a grant from the National Science Foundation DMR-9724294. This research was carried out under grants EP/G068437/1 and EP/I022562/1 from the UK Engineering and Physical Sciences Research Council (EPSRC).; J.N.C. gratefully acknowledges financial support from the Volkswagen Foundation. NR 30 TC 3 Z9 3 U1 1 U2 23 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD MAR 9 PY 2015 VL 23 IS 5 BP 5452 EP 5467 DI 10.1364/OE.23.005452 PG 16 WC Optics SC Optics GA CD2BL UT WOS:000350878500008 PM 25836778 ER PT J AU Camacho-Bunquin, J Siladke, NA Zhang, GH Niklas, J Poluektov, OG Nguyen, ST Miller, JT Hock, AS AF Camacho-Bunquin, Jeffrey Siladke, Nathan A. Zhang, Guanghui Niklas, Jens Poluektov, Oleg G. Nguyen, SonBinh T. Miller, Jeffrey T. Hock, Adam S. TI Synthesis and Catalytic Hydrogenation Reactivity of a Chromium Catecholate Porous Organic Polymer SO ORGANOMETALLICS LA English DT Article ID SURFACE ORGANOMETALLIC CHEMISTRY; H BOND ACTIVATION; OLEFIN POLYMERIZATION; HETEROGENEOUS CATALYSIS; SINGLE-SITE; C-H; ETHYLENE OLIGOMERIZATION; HOMOGENEOUS CATALYSIS; ALKENE HYDROGENATION; SUPPORTED CHROMIUM AB A single-site chromium catecholate POP (catPOP A(2)B(1)) was synthesized and characterized via AT-IR, XAS, and EPR spectroscopy. The well-defined, four-coordinate, 11-electron Cr(III) centers bound to catecholate POP were demonstrated to be active hydrogenation catalysts for nonpolar unsaturated organic substrates under mild conditions (5 mol % of Cr, 200 psi of H-2, 60 degrees C). This material constitutes the first example of a well-defined, supported organometallic chromium hydrogenation precatalyst. C1 [Camacho-Bunquin, Jeffrey; Siladke, Nathan A.; Zhang, Guanghui; Niklas, Jens; Poluektov, Oleg G.; Nguyen, SonBinh T.; Miller, Jeffrey T.; Hock, Adam S.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Nguyen, SonBinh T.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Nguyen, SonBinh T.] Northwestern Univ, Int Inst Nanotechnol, Evanston, IL 60208 USA. [Hock, Adam S.] IIT, Dept Biol & Chem Sci, Chicago, IL 60616 USA. RP Hock, AS (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM ahock@iit.edu RI Zhang, Guanghui/C-4747-2008; Nguyen, SonBinh/C-1682-2014; BM, MRCAT/G-7576-2011; Niklas, Jens/I-8598-2016; Hock, Adam/D-7660-2012 OI Zhang, Guanghui/0000-0002-5854-6909; Nguyen, SonBinh/0000-0002-6977-3445; Niklas, Jens/0000-0002-6462-2680; Hock, Adam/0000-0003-1440-1473 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences [DE-AC02-06CH11357]; U.S. DOE [DE-AC02-06CH11357] FX The authors thank Dr. Kristine Tanabe for assistance in the GC analyses. This work was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences, under Contract DE-AC02-06CH11357. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. Materials Research Collaborative Access Team (MRCAT, Sector 10-BM) operations are supported by the Department of Energy and the MRCAT member institutions. NR 65 TC 5 Z9 5 U1 5 U2 37 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0276-7333 EI 1520-6041 J9 ORGANOMETALLICS JI Organometallics PD MAR 9 PY 2015 VL 34 IS 5 BP 947 EP 952 DI 10.1021/om501321t PG 6 WC Chemistry, Inorganic & Nuclear; Chemistry, Organic SC Chemistry GA CD1NI UT WOS:000350841200017 ER PT J AU Grigoriev, A Yang, C Azad, MM Causey, O Walko, DA Tinberg, DS Trolier-McKinstry, S AF Grigoriev, Alexei Yang, Chun Azad, Mandana Meisami Causey, Oliver Walko, Donald A. Tinberg, Daniel S. Trolier-McKinstry, Susan TI Piezoelectric and dielectric properties of Pb(Zr,Ti)O-3 ferroelectric bilayers SO PHYSICAL REVIEW B LA English DT Article ID THIN-FILMS; SUPERLATTICES AB The dielectric and piezoelectric properties of an epitaxial PbZr0.8Ti0.2O3/PbZr0.6Ti0.4O3 ferroelectric bilayer film were studied. Time-resolved synchrotron x-ray microdiffraction provided access to layer-specific structural information during electric-field-induced changes. The observed dielectric and electromechanical responses are consistent with a weak electrostatic polarization coupling and can be described using a thermodynamic model of epitaxial ferroelectric bilayers. The weak electrostatic coupling between ferroelectric layers can enable unusual tail-to-tail and head-to-head polarization configurations. X-ray measurements of the piezoelectric response of the ferroelectric bilayer at a microsecond time scale confirmed a possible tail-to-tail polarization domain configuration. C1 [Grigoriev, Alexei; Yang, Chun; Azad, Mandana Meisami; Causey, Oliver] Univ Tulsa, Dept Phys & Engn Phys, Tulsa, OK 74104 USA. [Walko, Donald A.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Tinberg, Daniel S.; Trolier-McKinstry, Susan] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. RP Grigoriev, A (reprint author), Univ Tulsa, Dept Phys & Engn Phys, Tulsa, OK 74104 USA. EM alexei-grigoriev@utulsa.edu OI Trolier-McKinstry, Susan/0000-0002-7267-9281 FU NSF DMR [DMR-1057159]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work was supported by the NSF DMR (Award No. DMR-1057159). The use of the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 36 TC 1 Z9 1 U1 1 U2 15 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD MAR 9 PY 2015 VL 91 IS 10 AR 104106 DI 10.1103/PhysRevB.91.104106 PG 6 WC Physics, Condensed Matter SC Physics GA CC8LM UT WOS:000350620200003 ER PT J AU Wu, JJ Sato, T Lee, TSH AF Wu, Jia-Jun Sato, T. Lee, T. -S. H. TI Incoherent pion production in neutrino-deuteron interactions SO PHYSICAL REVIEW C LA English DT Article ID CROSS-SECTIONS; SCATTERING; SINGLE; PHOTOPRODUCTION; HYDROGEN; NUCLEI AB Within the multiple scattering formulation, the incoherent pion production in neutrino-deuteron reactions at energies near the Delta(1232) resonance is investigated. The calculations include an impulse term and one-loop contributions from nucleon-nucleon (NN) and pion-nucleon (pi N) final-state interactions. The input amplitudes of pi N scattering and electroweak pion-production reaction on the nucleon are generated from a dynamical model, which describes very extensive data of pi N scattering and both the electromagnetic and the weak pion-production reactions on the nucleon. The NN scattering amplitudes are generated from the Bonn potential. The validity of the calculational procedures is established by giving a reasonably good description of the data of pion photoproduction on the deuteron. The constructed model is then applied to predict the cross sections of nu + d -> mu(-) + pi(+) + n + p and nu + d -> mu(-) + pi(0) + p + p reactions. The importance of including the NN final-state interactions to understand the experimental data of these neutrino-deuteron reactions is demonstrated. Our results strongly suggest that the spectator approximation used in the previous analyses to extract the pion-production cross sections on the nucleon from the data on the deuteron is not valid for the nu + d -> mu(-) + pi(+) + n + p, but is a good approximation for nu + d -> mu(-) + pi(0) + p + p. C1 [Wu, Jia-Jun; Lee, T. -S. H.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Sato, T.] Osaka Univ, Dept Phys, Toyonaka, Osaka 5600043, Japan. RP Wu, JJ (reprint author), Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. FU U.S. Department of Energy, Office of Nuclear Physics Division [DE-AC02-06CH11357]; Japan Society for the Promotion of Science (JSPS) KAKENHI [24540273, 25105010]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX We thank B. Krusche for his help in explaining the data of Ref. [43]. This work was supported by the U.S. Department of Energy, Office of Nuclear Physics Division, under Contract No. DE-AC02-06CH11357, and the Japan Society for the Promotion of Science (JSPS) KAKENHI Grants No. 24540273 and No. 25105010. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231, and resources provided on the Blues and/or Fusion high-performance computing cluster operated by the Laboratory Computing Resource Center at Argonne National Laboratory. NR 50 TC 8 Z9 8 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD MAR 9 PY 2015 VL 91 IS 3 AR 035203 DI 10.1103/PhysRevC.91.035203 PG 11 WC Physics, Nuclear SC Physics GA CC8MJ UT WOS:000350622500006 ER PT J AU Burdman, G Chacko, Z Harnik, R de Lima, L Verhaaren, CB AF Burdman, Gustavo Chacko, Zackaria Harnik, Roni de Lima, Leonardo Verhaaren, Christopher B. TI Colorless top partners, a 125 GeV Higgs boson, and the limits on naturalness SO PHYSICAL REVIEW D LA English DT Article ID ELECTROWEAK SYMMETRY-BREAKING; STANDARD MODEL; ATLAS DETECTOR; PP COLLISIONS; SEARCH; LHC AB Theories of physics beyond the standard model that address the hierarchy problem generally involve top partners, new particles that cancel the quadratic divergences associated with the Yukawa coupling of the Higgs boson to the top quark. With extensions of the standard model that involve new colored particles coming under strain from collider searches, scenarios in which the top partners carry no charge under the strong interactions have become increasingly compelling. Although elusive for direct searches, these theories predict modified couplings of the Higgs boson to the standard model particles. This results in corrections to the Higgs production and decay rates that can be detected at the LHC provided the top partners are sufficiently light, and the theory correspondingly natural. In this paper we consider three theories that address the little hierarchy problem and involve colorless top partners, specifically the mirror twin Higgs, folded supersymmetry, and the quirky little Higgs. For each model we investigate the current and future bounds on the top partners, and the corresponding limits on naturalness, that can be obtained from the Higgs program at the LHC. We conclude that the LHC will not be able to strongly disfavor naturalness, with mild tuning at the level of about one part in ten remaining allowed even with 3000 fb(-1) of data at 14 TeV. C1 [Burdman, Gustavo] Univ Sao Paulo, Inst Fis, BR-05508900 Sao Paulo, Brazil. [Chacko, Zackaria; Verhaaren, Christopher B.] Univ Maryland, Maryland Ctr Fundamental Phys, Dept Phys, College Pk, MD 20742 USA. [Harnik, Roni] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [de Lima, Leonardo] Univ Estadual Paulista, Inst Fis Teor, BR-01140070 Sao Paulo, Brazil. RP Burdman, G (reprint author), Univ Sao Paulo, Inst Fis, BR-05508900 Sao Paulo, Brazil. FU National Science Foundation (NSF) [PHY-1315155]; United States Department of Energy [DE-AC02-07CH11359]; National Science Foundation [PHYS-1066293]; State of Sao Paulo Research Foundation (FAPESP); Brazilian National Council for Technological and Scientific Development (CNPq) FX We thank Reinard Primulando and Tien-Tien Yu for discussions during early stages of this work. Z. C. and C. V. are supported by the National Science Foundation (NSF) Grant No. PHY-1315155. Fermilab is operated by Fermi Research Alliance, LLC, under Contract No. DE-AC02-07CH11359 with the United States Department of Energy. R. H.'s work was supported in part by the National Science Foundation under Grant No. PHYS-1066293 and the hospitality of the Aspen Center for Physics. G. B. and L. L. acknowledge the support of the State of Sao Paulo Research Foundation (FAPESP). G. B. thanks the Brazilian National Council for Technological and Scientific Development (CNPq) for partial support and the University of Maryland Particle Theory group for its hospitality. NR 39 TC 33 Z9 33 U1 0 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD MAR 9 PY 2015 VL 91 IS 5 AR 055007 DI 10.1103/PhysRevD.91.055007 PG 15 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA CC8MR UT WOS:000350623300003 ER EF