FN Thomson Reuters Web of Science™ VR 1.0 PT J AU Kim, J Yoo, G Lee, H Lim, J Kim, K Kim, CW Park, MS Yang, JW AF Kim, Jungmin Yoo, Gursong Lee, Hansol Lim, Juntaek Kim, Kyochan Kim, Chul Woong Park, Min S. Yang, Ji-Won TI Methods of downstream processing for the production of biodiesel from microalgae SO BIOTECHNOLOGY ADVANCES LA English DT Review DE Biodiesel; Downstream process; Extraction; Harvest; Microalgae; Transesterification ID ALGA BOTRYOCOCCUS-BRAUNII; SYNECHOCYSTIS PCC 6803; CHLORELLA-VULGARIS; LIPID EXTRACTION; CELL-DISRUPTION; VEGETABLE-OILS; SUPERCRITICAL METHANOL; ULTRASONIC CAVITATION; MAGNETIC SEPARATION; ASSISTED EXTRACTION AB Despite receiving increasing attention during the last few decades, the production of microalgal biofuels is not yet sufficiently cost-effective to compete with that of petroleum-based conventional fuels. Among the steps required for the production of microalgal biofuels, the harvest of the microalgal biomass and the extraction of lipids from microalgae are two of the most expensive. In this review article, we surveyed a substantial amount of previous work in microalgal harvesting and lipid extraction to highlight recent progress in these areas. We also discuss new developments in the biodiesel conversion technology due to the importance of the connectivity of this step with the lipid extraction process. Furthermore, we propose possible future directions for technological or process improvements that will directly affect the final production costs of microalgal biomass-based biofuels. (C) 2013 Elsevier Inc. All rights reserved. C1 [Kim, Jungmin; Yoo, Gursong; Lee, Hansol; Lim, Juntaek; Kim, Kyochan; Kim, Chul Woong; Park, Min S.; Yang, Ji-Won] Korea Adv Inst Sci & Technol, Dept Chem & Biomol Engn, Taejon 305701, South Korea. [Lim, Juntaek; Park, Min S.; Yang, Ji-Won] Korea Adv Inst Sci & Technol, Adv Biomass R&D Ctr, Taejon 305701, South Korea. [Park, Min S.] Los Alamos Natl Lab, Biosci Div, Los Alamos, NM 87545 USA. RP Park, MS (reprint author), Korea Adv Inst Sci & Technol, Adv Biomass R&D Ctr, 291 Daehak Ro, Taejon 305701, South Korea. EM minsungpark0@kaist.ac.kr; jwyang@kaist.ac.kr RI Yang, Ji-Won/C-1933-2011; OI Kim, Jungmin/0000-0002-8580-8134 FU Advanced Biomass R&D Center (ABC) of Global Frontier Project; Ministry of Education, Science and Technology [ABC-2011-K000908]; National Energy Technology Innovation of the Korea Institute of Energy Technology Evaluation and Planning (KETEP) grant; Korea government Ministry of Knowledge Economy [2012 T100201665]; Brain Pool Program; Korean Federation of Science and Technology Societies Grant by Korea Government (MEST, Basic Research Promotion Fund) FX This work was supported by the Advanced Biomass R&D Center (ABC) of Global Frontier Project funded by the Ministry of Education, Science and Technology (ABC-2011-K000908). This work was also supported by the National Energy Technology Innovation of the Korea Institute of Energy Technology Evaluation and Planning (KETEP) grant funded by the Korea government Ministry of Knowledge Economy (No. 2012 T100201665). MSP was supported by the Brain Pool Program funded by the Korean Federation of Science and Technology Societies Grant by Korea Government (MEST, Basic Research Promotion Fund). NR 116 TC 106 Z9 108 U1 12 U2 371 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0734-9750 J9 BIOTECHNOL ADV JI Biotechnol. Adv. PD NOV 1 PY 2013 VL 31 IS 6 SI SI BP 862 EP 876 DI 10.1016/j.biotechadv.2013.04.006 PG 15 WC Biotechnology & Applied Microbiology SC Biotechnology & Applied Microbiology GA 217IH UT WOS:000324352700012 PM 23632376 ER PT J AU Hansen, N Merchant, SS Harper, MR Green, WH AF Hansen, Nils Merchant, Shamel S. Harper, Michael R. Green, William H. TI The predictive capability of an automatically generated combustion chemistry mechanism: Chemical structures of premixed iso-butanol flames SO COMBUSTION AND FLAME LA English DT Article DE iso-Butanol; Chemical mechanism; Mass spectrometry; Premixed flame ID PHOTOIONIZATION MASS-SPECTROMETRY; JET-STIRRED REACTOR; MASTER EQUATION METHODS; LOW-PRESSURE FLAMES; N-BUTANOL; SHOCK-TUBE; CROSS-SECTIONS; GAS-PHASE; OXIDATION; KINETICS AB The chemical compositions of four low-pressure premixed flames of iso-butanol are investigated with an emphasis on assessing the predictive capabilities of an automatically generated combustion chemistry model. This kinetic model had been extensively tested against earlier experimental data [S.S. Merchant, E.F. Zanoelo, R.L. Speth, M.R. Harper, K.M. Van Geem, W.H. Green, Combust. Flame (2013), http://dx.doLorg/10.1016/j.combustflame.2013.04.023.] and also shows impressive capabilities for predicting the new flame data presented here. The new set of data consists of isomer-resolved mole fraction profiles for more than 40 species in each of the four flames and provides a comprehensive benchmark for testing of any combustion chemistry model for iso-butanol. Isomer-specificity is achieved by analyzing flames, which are burner-stabilized at equivalence ratios of phi = 1.0-1.5 and at pressures between 15 and 30 Torr, with molecular-beam mass spectrometry and single-photon ionization by tunable vacuum-ultraviolet synchrotron radiation. Predictions of the C2H4O, C3H6O, and C4H8O enol-aldehyde-ketone isomers are improved compared to the earlier work by Hansen et al. [N. Hansen, M. R. Harper, W. H. Green, Phys. Chem. Chem. Phys. 13 (2011) 20262-20274] on similar n-butanol flames. A reaction path analysis identifies prominent fuel-consumption and oxidation sequences. Almost all of the species mole fraction data reported here are predicted within the measurement uncertainties of a factor of two to three. Some significant differences with previous published models are highlighted. (C) 2013 The Combustion Institute. Published by Elsevier Inc. All rights reserved. C1 [Hansen, Nils] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA. [Merchant, Shamel S.; Harper, Michael R.; Green, William H.] MIT, Dept Chem Engn, Cambridge, MA 02139 USA. RP Hansen, N (reprint author), Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA. EM nhansen@sandia.gov; whgreen@mit.edu RI Green, William/C-9684-2012; Hansen, Nils/G-3572-2012 OI Green, William/0000-0003-2603-9694; FU U.S. Department of Energy, Office of Basic Energy Sciences under the Energy Frontier Research Center for Combustion Science [DE-SC0001198]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; National Nuclear Security Administration [DE-AC04-94-AL85000] FX The work is supported by the U.S. Department of Energy, Office of Basic Energy Sciences under the Energy Frontier Research Center for Combustion Science (Grant No. DE-SC0001198). The authors thank P. Osswald, K. Kohse-Hoinghaus, and F. Qi for sharing their temperature and speciation data. SSM thanks Dr. Judit Zador and Dr. J. A. Miller for sharing their recent calculations on the propene + OH potential energy surface. The measurements are performed within the "Flame Team" collaboration at the Advanced Light Source (ALS), Lawrence Berkeley National Laboratory, Berkeley, USA, and we thank the students and postdocs for the help with the data acquisition. The experiments have profited from the expert technical assistance of Paul Fugazzi. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Sandia is a multi-program laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the National Nuclear Security Administration under Contract DE-AC04-94-AL85000. NR 65 TC 21 Z9 21 U1 5 U2 67 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 0010-2180 J9 COMBUST FLAME JI Combust. Flame PD NOV PY 2013 VL 160 IS 11 BP 2343 EP 2351 DI 10.1016/j.combustflame.2013.05.013 PG 9 WC Thermodynamics; Energy & Fuels; Engineering, Multidisciplinary; Engineering, Chemical; Engineering, Mechanical SC Thermodynamics; Energy & Fuels; Engineering GA 212TT UT WOS:000324006400005 ER PT J AU Chatakonda, O Hawkes, ER Aspden, AJ Kerstein, AR Kolla, H Chen, JH AF Chatakonda, Obulesu Hawkes, Evatt R. Aspden, Andrew J. Kerstein, Alan R. Kolla, Hemanth Chen, Jacqueline H. TI On the fractal characteristics of low Damkohler number flames SO COMBUSTION AND FLAME LA English DT Article DE Turbulent premixed combustion; Fractal; Fractal dimension; Inner cut-off; Direct numerical simulation; Large-eddy simulation ID PREMIXED TURBULENT COMBUSTION; LARGE-EDDY SIMULATION; DIRECT NUMERICAL SIMULATIONS; PLANE JET FLAMES; SURFACE-DENSITY; IA SUPERNOVAE; DYNAMIC FORMULATION; BURNING VELOCITY; WRINKLING MODEL; HEATED COFLOW AB Knowledge of the fractal properties of premixed flame surfaces can potentially be used to help develop turbulent combustion models. Here, direct numerical simulations of low Damkohler number flames are used to analyse the fractal nature of the flames. Two sets of data are considered: (i) thermochemical hydrogen-air turbulent premixed plane-jet flames with detailed chemistry and (ii) thermonuclear flames in type la supernovae. A three-dimensional box counting method is used to investigate fractal dimension of the flame surface, characterising the self similarity of flame fronts. In the premixed flames, the fractal dimension is found to vary in time between 2.1 and 2.7. The supernovae flames in distributed combustion regimes yield fractal dimension about 2.7. The results for the maximum fractal dimensions are higher than previously reported. They are explained theoretically by a Reynolds number similarity argument which posits that the high Reynolds number, low Damkohler number limiting value of the fractal dimension is 8/3. Also tested is Mandelbrot's fractal additive law which relates the fractal dimension determined in two dimensions, which is typical of experimental measurements, to that in three dimensions. The comparison of the fractal dimension in both two-dimensional and three-dimensional spaces supports the additive law, even though the flames considered do not formally satisfy isotropy. Finally, the inner-cut off is extracted from the hydrogen flames and found to be consistent in order of magnitude with Kolmogorov scaling. (C) 2013 The Combustion Institute. All rights reserved. C1 [Chatakonda, Obulesu; Hawkes, Evatt R.] Univ New S Wales, Sch Photovolta & Renewable Energy Engn, Sydney, NSW 2052, Australia. [Hawkes, Evatt R.] Univ New S Wales, Sch Mech & Mfg Engn, Sydney, NSW 2052, Australia. [Aspden, Andrew J.] Univ Portsmouth, Sch Engn, Portsmouth PO1 3DJ, Hants, England. [Kerstein, Alan R.; Kolla, Hemanth; Chen, Jacqueline H.] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA. RP Hawkes, ER (reprint author), Univ New S Wales, Sch Photovolta & Renewable Energy Engn, Sydney, NSW 2052, Australia. EM evatt.hawkes@unsw.edu.au RI Kolla, Hemanth/L-2142-2013; Aspden, Andy/A-7391-2017; Hawkes, Evatt/C-5307-2012 OI Kolla, Hemanth/0000-0003-4969-5870; Aspden, Andy/0000-0002-2970-4824; Hawkes, Evatt/0000-0003-0539-7951 FU Australian Research Council [FT100100536]; Office of Science of the U.S. Department of Energy [DEAC05-00OR22725] FX This work was supported by the Australian Research Council under Grant No. FT100100536. The research used resources of the Oak Ridge Leadership Computing Facility at the Oak Ridge National Laboratory, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DEAC05-00OR22725, and the resources of the National Computational Infrastructure, Australia through the National Merit Allocation Scheme and the Intersect, Australia partner share. NR 73 TC 20 Z9 21 U1 0 U2 36 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 0010-2180 J9 COMBUST FLAME JI Combust. Flame PD NOV PY 2013 VL 160 IS 11 BP 2422 EP 2433 DI 10.1016/j.combustflame.2013.05.007 PG 12 WC Thermodynamics; Energy & Fuels; Engineering, Multidisciplinary; Engineering, Chemical; Engineering, Mechanical SC Thermodynamics; Energy & Fuels; Engineering GA 212TT UT WOS:000324006400012 ER PT J AU Coriton, B Frank, JH Gomez, A AF Coriton, Bruno Frank, Jonathan H. Gomez, Alessandro TI Effects of strain rate, turbulence, reactant stoichiometry and heat losses on the interaction of turbulent premixed flames with stoichiometric counterflowing combustion products SO COMBUSTION AND FLAME LA English DT Article DE Turbulent premixed flames; Extinction; Ignition; Counterflow; Strain rate; Heat loss ID OPPOSED-JET FLAMES; LARGE-EDDY SIMULATION; BURNING RATE; FLOW-FIELD; AIR FLAMES; EXTINCTION; VELOCITY; CHEMISTRY; STREAMS; CURVATURE AB Intense strain, turbulence, heat transfer, and mixing with combustion products can affect premixed flames in practical combustion devices. These effects are systematically studied in turbulent premixed CH4/N-2/O-2 flames using a reactant versus product counterflow system and independently varying bulk strain rate, turbulent Reynolds number, equivalence ratio of the reactant mixture, and temperature of the stoichiometric counterflowing combustion products. The flow field and the turbulent flames are investigated using particle image velocimetry (PIV) measurements and laser-induced fluorescence (LIF) imaging of OH. The OH-LIF images are used to identify the interface between the counterflowing streams, referred to here as the gas mixing layer interface (GMLI). The flame response for different flow conditions is compared in terms of the probability of localized extinction along the GMLI, the turbulent flame brush thickness, and flame position relative to the GMLI, by using an OH-LIF-based progress variable. The probability of localized extinction at the GMLI increases as the separation between the turbulent flame brush and the GMLI decreases. Flame fronts in the vicinity of the GMLI are more likely to extinguish as a result of heat losses, dilution of the reaction zone by the product stream, and large local strain rates. A higher probability of localized extinction at the GMLI is induced by either a larger bulk strain rate or a slower flame speed. As the turbulent Reynolds number increases, the corresponding increase in turbulent flame brush thickness enhances the interactions of the flame fronts with the GMLI. Heat losses are substantially less significant for cases in which the turbulent flame brush is sufficiently separated from the GMLI. For flames in close proximity to the GMLI, the effects of the product stream on the flame front differ for lean and rich reactant mixtures. These disparities are attributed in part to differences in the ignitibility of the reactant mixtures by the hot product stream. (C) 2013 The Combustion Institute. Published by Elsevier Inc. All rights reserved. C1 [Coriton, Bruno; Frank, Jonathan H.] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA. [Gomez, Alessandro] Yale Univ, Dept Mech Engn & Mat Sci, Yale Ctr Combust Studies, New Haven, CT 06520 USA. RP Gomez, A (reprint author), Yale Univ, Dept Mech Engn & Mat Sci, Yale Ctr Combust Studies, New Haven, CT 06520 USA. EM alessandro.gomez@yale.edu FU American Chemical Society (ACS) [46991-AC9]; NSF [1060762.1.D1692.652001]; US Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences; US Department of Energy [DE-AC04-94-AL85000] FX The authors gratefully acknowledge the support of the American Chemical Society (ACS) through Grant PRF#46991-AC9 and of NSF (Grant #1060762.1.D1692.652001, Drs. Arvind Atreya and Ruey-Hung Chen, Program Directors) and the US Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences. Sandia National Laboratories is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the US Department of Energy under Contract DE-AC04-94-AL85000. NR 55 TC 15 Z9 16 U1 4 U2 49 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 0010-2180 J9 COMBUST FLAME JI Combust. Flame PD NOV PY 2013 VL 160 IS 11 BP 2442 EP 2456 DI 10.1016/j.combustflame.2013.05.009 PG 15 WC Thermodynamics; Energy & Fuels; Engineering, Multidisciplinary; Engineering, Chemical; Engineering, Mechanical SC Thermodynamics; Energy & Fuels; Engineering GA 212TT UT WOS:000324006400014 ER PT J AU Cooper, MA Oliver, MS AF Cooper, Marcia A. Oliver, Michael S. TI The burning regimes and conductive burn rates of titanium subhydride potassium perchlorate (TiH1.65/KClO4) in hybrid closed bomb-strand burner experiments SO COMBUSTION AND FLAME LA English DT Article DE Pyrotechnic; Strand burner; Closed bomb; Conductive burning; Conductive-to-convective transition AB A hybrid closed bomb-strand burner is used to measure the burning behavior of the titanium subhydride potassium perchlorate pyrotechnic with an equivalent hydrogen concentration of 1.65. This experimental facility allows for simultaneous measurement of the closed bomb pressure rise and pyrotechnic burn rate as detected by electrical break wires over a range of pressures. Strands were formed by pressing the pyrotechnic powders to bulk solid volume fractions between 0.58 and 0.88 theoretical maximum density. The burn rate dependence on average pressed powder density and initial vessel pressure are measured. Data from the strands with a 0.68 theoretical maximum density are compared to available literature. At all initial strand densities, the burn is observed to transition from a steady conductive burn to an unsteady convective burn within the strand. The conductive burning regime is analyzed following traditional closed bomb methods used with propellants and incorporating a relevant instantaneous burning surface area for the pyrotechnic powder bed. The transition to convective burning is analyzed and a relationship between the initial material characteristics of the pyrotechnic powder bed and the critical pressure at transition is developed. (c) 2013 The Combustion Institute. All rights reserved. C1 [Cooper, Marcia A.; Oliver, Michael S.] Sandia Natl Labs, Explos Technol Grp, Albuquerque, NM 87185 USA. EM macoope@sandia.gov FU Stockpile Weapons Research Program at Sandia National Laboratories; United States Department of Energys National Nuclear Security Administration [DE-AC04-94AL85000] FX This work has been funded by the Stockpile Weapons Research Program at Sandia National Laboratories. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed-Martin Company, for the United States Department of Energys National Nuclear Security Administration under Contract DE-AC04-94AL85000. NR 37 TC 2 Z9 2 U1 0 U2 12 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 0010-2180 J9 COMBUST FLAME JI Combust. Flame PD NOV PY 2013 VL 160 IS 11 BP 2619 EP 2630 DI 10.1016/j.combustflame.2013.05.015 PG 12 WC Thermodynamics; Energy & Fuels; Engineering, Multidisciplinary; Engineering, Chemical; Engineering, Mechanical SC Thermodynamics; Energy & Fuels; Engineering GA 212TT UT WOS:000324006400029 ER PT J AU Su, D Gaffrey, MJ Guo, J Clauss, TRW Thrall, BD Smith, RD Qian, WJ AF Su, Dian Gaffrey, Matthew J. Guo, Jia Clauss, Therese R. W. Thrall, Brian D. Smith, Richard D. Qian, Wei-Jun TI A General Proteomics Approach for Site-Specific Quantification of Cysteine Redox Modifications and Its Application for Profiling S-Glutathionylation in Macrophages SO FREE RADICAL BIOLOGY AND MEDICINE LA English DT Meeting Abstract C1 [Su, Dian; Gaffrey, Matthew J.; Guo, Jia; Clauss, Therese R. W.; Thrall, Brian D.; Smith, Richard D.; Qian, Wei-Jun] Pacific NW Natl Lab, Richland, WA 99352 USA. RI Smith, Richard/J-3664-2012 OI Smith, Richard/0000-0002-2381-2349 NR 0 TC 0 Z9 0 U1 0 U2 0 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 0891-5849 EI 1873-4596 J9 FREE RADICAL BIO MED JI Free Radic. Biol. Med. PD NOV 1 PY 2013 VL 65 SU 2 MA 356 BP S152 EP S153 DI 10.1016/j.freeradbiomed.2013.10.782 PG 2 WC Biochemistry & Molecular Biology; Endocrinology & Metabolism SC Biochemistry & Molecular Biology; Endocrinology & Metabolism GA V40JU UT WOS:000209475700374 ER PT J AU Moyer, JA Kumah, DP Vaz, CAF Arena, DA Henrich, VE AF Moyer, J. A. Kumah, D. P. Vaz, C. A. F. Arena, D. A. Henrich, V. E. TI Role of epitaxial strain on the magnetic structure of Fe-doped CoFe2O4 SO JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS LA English DT Article DE Iron-doped cobalt ferrite; Magnetic structure; Molecular beam epitaxy; Epitaxial strain ID TRANSITION-METAL COMPOUNDS; FERRITE THIN-FILMS; RAY CIRCULAR-DICHROISM; 2P ABSORPTION-SPECTRA; COBALT FERRITE; ANISOTROPY; ORIGIN; FE3O4; NANOSTRUCTURES; BEHAVIOR AB The magnetic structure of Fe-doped CoFe2O4 (Co1-xFe2+xO4) grown on MgO (0 0 1) and SrTiO3 (0 0 1) substrates is studied with superconducting quantum interference device magnetometry and soft x-ray magnetic spectroscopies. X-ray and electron diffraction show that the choice of substrate has large effects on the strain, crystal structure and surface morphology of Co1-xFe2+xO4 thin films. Samples grown on MgO have small, coherent strains and surfaces that are nearly atomically flat, whereas films grown on SrTiO3 have large tensile strains and surfaces terminated with islands, which indicate the presence of a large density of misfit dislocations. These differences in structural properties correlate with the large differences seen in the magnetic structure; samples grown on SrTiO3 have larger magnetic moments and increased anisotropies compared to those grown on MgO. Most strikingly, the large magnetic spin and orbital moments found in the films grown on SrTiO3 suggest a suppression of anti-phase boundary formation, which we attribute to the large compressive lattice mismatch and the formation of misfit dislocations during the film growth in order to relieve the epitaxial strain. This results in the films grown on SrTiO3 having magnetic properties that are more similar to bulk Co1-xFe2+xO4 than those grown on MgO, demonstrating that epitaxial strain can result in large changes in the magnetic structure of Co1-xFe2+xO4. (C) 2013 Elsevier B.V. All rights reserved. C1 [Moyer, J. A.; Kumah, D. P.; Henrich, V. E.] Yale Univ, Dept Appl Phys, New Haven, CT 06511 USA. [Moyer, J. A.; Kumah, D. P.; Henrich, V. E.] Yale Univ, Ctr Res Interface Struct & Phenomena, New Haven, CT 06511 USA. [Vaz, C. A. F.] Paul Scherrer Inst, SwissFEL, CH-5232 Villigen, Switzerland. [Arena, D. A.] Brookhaven Natl Lab, Natl Synchrotron Light Source, Upton, NY 11973 USA. RP Moyer, JA (reprint author), Univ Illinois, Dept Phys, Urbana, IL 61801 USA. EM moyerja@illinois.edu RI Vaz, Carlos/A-7240-2012; Kumah, Divine/A-7031-2011 OI Vaz, Carlos/0000-0002-6209-8918; Kumah, Divine/0000-0003-0715-1285 FU NSF through MRSEC [DMR 1119826 (CRISP)]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX The authors acknowledge primary financial support by the NSF through MRSEC DMR 1119826 (CRISP). Use of the National Synchrotron Light Source, Brookhaven National Laboratory, was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. NR 44 TC 5 Z9 5 U1 3 U2 80 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0304-8853 J9 J MAGN MAGN MATER JI J. Magn. Magn. Mater. PD NOV PY 2013 VL 345 BP 180 EP 189 DI 10.1016/j.jmmm.2013.06.031 PG 10 WC Materials Science, Multidisciplinary; Physics, Condensed Matter SC Materials Science; Physics GA 213HB UT WOS:000324045300032 ER PT J AU Bell, CW Fricks, BE Rocca, JD Steinweg, JM McMahon, SK Wallenstein, MD AF Bell, Colin W. Fricks, Barbara E. Rocca, Jennifer D. Steinweg, Jessica M. McMahon, Shawna K. Wallenstein, Matthew D. TI High-throughput Fluorometric Measurement of Potential Soil Extracellular Enzyme Activities SO JOVE-JOURNAL OF VISUALIZED EXPERIMENTS LA English DT Article DE Environmental Sciences; Issue 81; Ecological and Environmental Phenomena; Environment; Biochemistry; Environmental Microbiology; Soil Microbiology; Ecology; Eukaryota; Archaea; Bacteria; Soil extracellular enzyme activities (EEAs); fluorometric enzyme assays; substrate degradation; 4-methylumbelliferone (MUB); 7-amino-4-methylcoumarin (MUC); enzyme temperature kinetics; soil AB Microbes in soils and other environments produce extracellular enzymes to depolymerize and hydrolyze organic macromolecules so that they can be assimilated for energy and nutrients. Measuring soil microbial enzyme activity is crucial in understanding soil ecosystem functional dynamics. The general concept of the fluorescence enzyme assay is that synthetic C-, N-, or P-rich substrates bound with a fluorescent dye are added to soil samples. When intact, the labeled substrates do not fluoresce. Enzyme activity is measured as the increase in fluorescence as the fluorescent dyes are cleaved from their substrates, which allows them to fluoresce. Enzyme measurements can be expressed in units of molarity or activity. To perform this assay, soil slurries are prepared by combining soil with a pH buffer. The pH buffer (typically a 50 mM sodium acetate or 50 mM Tris buffer), is chosen for the buffer's particular acid dissociation constant (pKa) to best match the soil sample pH. The soil slurries are inoculated with a nonlimiting amount of fluorescently labeled (i.e. C-, N-, or P-rich) substrate. Using soil slurries in the assay serves to minimize limitations on enzyme and substrate diffusion. Therefore, this assay controls for differences in substrate limitation, diffusion rates, and soil pH conditions; thus detecting potential enzyme activity rates as a function of the difference in enzyme concentrations (per sample). Fluorescence enzyme assays are typically more sensitive than spectrophotometric (i.e. colorimetric) assays, but can suffer from interference caused by impurities and the instability of many fluorescent compounds when exposed to light; so caution is required when handling fluorescent substrates. Likewise, this method only assesses potential enzyme activities under laboratory conditions when substrates are not limiting. Caution should be used when interpreting the data representing cross-site comparisons with differing temperatures or soil types, as in situ soil type and temperature can influence enzyme kinetics. C1 [Bell, Colin W.; Fricks, Barbara E.; Rocca, Jennifer D.; Wallenstein, Matthew D.] Colorado State Univ, Nat Resource Ecol Lab, Ft Collins, CO 80523 USA. [Steinweg, Jessica M.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN USA. [McMahon, Shawna K.] Univ Colorado, Dept Bioengn, Boulder, CO 80309 USA. RP Wallenstein, MD (reprint author), Colorado State Univ, Nat Resource Ecol Lab, Ft Collins, CO 80523 USA. EM matthew.wallenstein@colostate.edu RI Wallenstein, Matthew/C-6441-2008 OI Wallenstein, Matthew/0000-0002-6219-1442 FU Enzymes in the Environment Research Coordination Network Research - US National Science Foundation [1021559]; US National Science Foundation [1021559]; US Department of Energy's Office of Science (Biological and Environmental Research) FX This publication was funded by the Enzymes in the Environment Research Coordination Network Research supported by the US National Science Foundation (DEB# 1021559). This research was supported by the US National Science Foundation (DEB# 1021559), and the US Department of Energy's Office of Science (Biological and Environmental Research). Any opinions, findings, and conclusions or recommendations expressed in this material are those of the authors and do not necessarily reflect the views of the US NSF. NR 50 TC 14 Z9 14 U1 10 U2 46 PU JOURNAL OF VISUALIZED EXPERIMENTS PI CAMBRIDGE PA 1 ALEWIFE CENTER, STE 200, CAMBRIDGE, MA 02140 USA SN 1940-087X J9 JOVE-J VIS EXP JI J. Vis. Exp. PD NOV PY 2013 IS 81 AR UNSP e50961 DI 10.3791/50961 PG 16 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA V36RQ UT WOS:000209228900060 PM 24299913 ER PT J AU Doeff, MM Chen, GY Cabana, J Richardson, TJ Mehta, A Shirpour, M Duncan, H Kim, C Kam, KC Conry, T AF Doeff, Marca M. Chen, Guoying Cabana, Jordi Richardson, Thomas J. Mehta, Apurva Shirpour, Mona Duncan, Hugues Kim, Chunjoong Kam, Kinson C. Conry, Thomas TI Characterization of Electrode Materials for Lithium Ion and Sodium Ion Batteries Using Synchrotron Radiation Techniques SO JOVE-JOURNAL OF VISUALIZED EXPERIMENTS LA English DT Article DE Physics; Issue 81; X-Ray Absorption Spectroscopy; X-Ray Diffraction; inorganic chemistry; electric batteries (applications); energy storage; Electrode materials; Li-ion battery; Na-ion battery; X-ray Absorption Spectroscopy (XAS); in situ X-ray diffraction (XRD) AB Intercalation compounds such as transition metal oxides or phosphates are the most commonly used electrode materials in Li-ion and Na-ion batteries. During insertion or removal of alkali metal ions, the redox states of transition metals in the compounds change and structural transformations such as phase transitions and/or lattice parameter increases or decreases occur. These behaviors in turn determine important characteristics of the batteries such as the potential profiles, rate capabilities, and cycle lives. The extremely bright and tunable x-rays produced by synchrotron radiation allow rapid acquisition of high-resolution data that provide information about these processes. Transformations in the bulk materials, such as phase transitions, can be directly observed using X-ray diffraction (XRD), while X-ray absorption spectroscopy (XAS) gives information about the local electronic and geometric structures (e.g. changes in redox states and bond lengths). In situ experiments carried out on operating cells are particularly useful because they allow direct correlation between the electrochemical and structural properties of the materials. These experiments are time-consuming and can be challenging to design due to the reactivity and air-sensitivity of the alkali metal anodes used in the half-cell configurations, and/or the possibility of signal interference from other cell components and hardware. For these reasons, it is appropriate to carry out ex situ experiments (e.g. on electrodes harvested from partially charged or cycled cells) in some cases. Here, we present detailed protocols for the preparation of both ex situ and in situ samples for experiments involving synchrotron radiation and demonstrate how these experiments are done. C1 [Doeff, Marca M.; Chen, Guoying; Cabana, Jordi; Richardson, Thomas J.; Shirpour, Mona; Duncan, Hugues; Kim, Chunjoong] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Cabana, Jordi] Univ Illinois, Dept Chem, Chicago, IL 60680 USA. [Mehta, Apurva] Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA USA. [Kam, Kinson C.] Haldor Topsoe Res Labs, Ravnholm, Denmark. [Conry, Thomas] PolyPlus Battery Co, Berkeley, CA USA. RP Doeff, MM (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. EM mmdoeff@lbl.gov RI Cabana, Jordi/G-6548-2012 OI Cabana, Jordi/0000-0002-2353-5986 FU Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy [DE-AC02-05CH11231]; DOE Office of Biological and Environmental Research; National Institutes of Health, National Center for Research Resources, Biomedical Technology Program [P41RR001209] FX This work is supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Portions of this research were carried out at the Stanford Synchrotron Radiation Lightsource, a Directorate of SLAC National Accelerator Laboratory and an Office of Science User Facility operated for the U.S. Department of Energy Office of Science by Stanford University. The SSRL Structural Molecular Biology Program is supported by the DOE Office of Biological and Environmental Research, and by the National Institutes of Health, National Center for Research Resources, Biomedical Technology Program (P41RR001209). NR 22 TC 2 Z9 2 U1 8 U2 31 PU JOURNAL OF VISUALIZED EXPERIMENTS PI CAMBRIDGE PA 1 ALEWIFE CENTER, STE 200, CAMBRIDGE, MA 02140 USA SN 1940-087X J9 JOVE-J VIS EXP JI J. Vis. Exp. PD NOV PY 2013 IS 81 AR UNSP e50594 DI 10.3791/50594 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA V36RQ UT WOS:000209228900011 PM 24300777 ER PT J AU Gutschow, C Marshall, Z AF Guetschow, Christian Marshall, Zachary TI Setting Limits on Supersymmetry Using Simplified Models SO JOVE-JOURNAL OF VISUALIZED EXPERIMENTS LA English DT Article DE Physics; Issue 81; high energy physics; particle physics; Supersymmetry; LHC; ATLAS; CMS; New Physics Limits; Simplified Models AB Experimental limits on supersymmetry and similar theories are difficult to set because of the enormous available parameter space and difficult to generalize because of the complexity of single points. Therefore, more phenomenological, simplified models are becoming popular for setting experimental limits, as they have clearer physical interpretations. The use of these simplified model limits to set a real limit on a concrete theory has not, however, been demonstrated. This paper recasts simplified model limits into limits on a specific and complete supersymmetry model, minimal supergravity. Limits obtained under various physical assumptions are comparable to those produced by directed searches. A prescription is provided for calculating conservative and aggressive limits on additional theories. Using acceptance and efficiency tables along with the expected and observed numbers of events in various signal regions, LHC experimental results can be recast in this manner into almost any theoretical framework, including nonsupersymmetric theories with supersymmetry-like signatures. C1 [Guetschow, Christian] UCL, Dept Phys & Astron, London WC1E 6BT, England. [Marshall, Zachary] CERN, CH-1211 Geneva 23, Switzerland. [Marshall, Zachary] Lawrence Berkeley Natl Lab, Phys Div, Berkeley, CA USA. RP Marshall, Z (reprint author), CERN, CH-1211 Geneva 23, Switzerland. EM zach.marshall@cern.ch NR 47 TC 0 Z9 0 U1 0 U2 0 PU JOURNAL OF VISUALIZED EXPERIMENTS PI CAMBRIDGE PA 1 ALEWIFE CENTER, STE 200, CAMBRIDGE, MA 02140 USA SN 1940-087X J9 JOVE-J VIS EXP JI J. Vis. Exp. PD NOV PY 2013 IS 81 AR UNSP e50419 DI 10.3791/50419 PG 14 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA V36RQ UT WOS:000209228900003 PM 24300306 ER PT J AU Krishna, KS Biswas, S Navin, CV Yamane, DG Miller, JT Kumar, CSSR AF Krishna, Katla Sai Biswas, Sanchita Navin, Chelliah V. Yamane, Dawit G. Miller, Jeffrey T. Kumar, Challa S. S. R. TI Millifluidics for Chemical Synthesis and Time-resolved Mechanistic Studies SO JOVE-JOURNAL OF VISUALIZED EXPERIMENTS LA English DT Article DE Bioengineering; Issue 81; Millifluidics; Millifluidic Device; Time-resolved Kinetics; Synthesis; Catalysis; Nanomaterials; Lab-on-a-Chip AB Procedures utilizing millifluidic devices for chemical synthesis and time-resolved mechanistic studies are described by taking three examples. In the first, synthesis of ultra-small copper nanoclusters is described. The second example provides their utility for investigating time resolved kinetics of chemical reactions by analyzing gold nanoparticle formation using in situ X-ray absorption spectroscopy. The final example demonstrates continuous flow catalysis of reactions inside millifluidic channel coated with nanostructured catalyst. C1 [Krishna, Katla Sai; Biswas, Sanchita; Navin, Chelliah V.; Yamane, Dawit G.; Kumar, Challa S. S. R.] Louisiana State Univ, CAMD, Baton Rouge, LA 70803 USA. [Krishna, Katla Sai; Biswas, Sanchita; Navin, Chelliah V.; Kumar, Challa S. S. R.] Louisiana State Univ, Ctr Atom Level Catalyst Design, Cain Dept Chem Engn, Baton Rouge, LA 70803 USA. [Navin, Chelliah V.] Louisiana State Univ, Dept Biol & Agr Engn, Baton Rouge, LA 70803 USA. [Miller, Jeffrey T.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Kumar, CSSR (reprint author), Louisiana State Univ, CAMD, Baton Rouge, LA 70803 USA. EM ckumar1@lsu.edu FU Center for Atomic Level Catalyst Design, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001058]; Board of Regents [LEQSF (2009-14)-EFRC-MATCH, LEDSF-EPS(2012)-OPT-IN-15]; Department of Energy; MRCAT member institutions; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; Institute for Atom-efficient Chemical Transformations (IACT), an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences FX This research work is supported as part of the Center for Atomic Level Catalyst Design, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number DE-SC0001058 and also supported by Board of Regents under grants award number LEQSF (2009-14)-EFRC-MATCH and LEDSF-EPS(2012)-OPT-IN-15. MRCAT operations are supported by the Department of Energy and the MRCAT member institutions. The use of the Advanced Photon Source at ANL is supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. Financial support for JTM was provided as part of the Institute for Atom-efficient Chemical Transformations (IACT), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. NR 24 TC 1 Z9 1 U1 1 U2 12 PU JOURNAL OF VISUALIZED EXPERIMENTS PI CAMBRIDGE PA 1 ALEWIFE CENTER, STE 200, CAMBRIDGE, MA 02140 USA SN 1940-087X J9 JOVE-J VIS EXP JI J. Vis. Exp. PD NOV PY 2013 IS 81 AR UNSP e50711 DI 10.3791/50711 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA V36RQ UT WOS:000209228900022 ER PT J AU Jeen, H Choi, WS Biegalski, MD Folkman, CM Tung, IC Fong, DD Freeland, JW Shin, D Ohta, H Chisholm, MF Lee, HN AF Jeen, Hyoungjeen Choi, Woo Seok Biegalski, Michael D. Folkman, Chad M. Tung, I-Cheng Fong, Dillon D. Freeland, John W. Shin, Dongwon Ohta, Hiromichi Chisholm, Matthew F. Lee, Ho Nyung TI Reversible redox reactions in an epitaxially stabilized SrCoOx oxygen sponge SO NATURE MATERIALS LA English DT Article ID FUEL-CELLS; MAGNETIC-PROPERTIES; OXIDE; SRCOO3-DELTA; SPECTROSCOPY; TEMPERATURE; PERFORMANCE; REDUCTION; DIFFUSION; TRANSPORT AB Fast, reversible redox reactions in solids at low temperatures without thermomechanical degradation are a promising strategy for enhancing the overall performance and lifetime of many energy materials and devices. However, the robust nature of the cation's oxidation state and the high thermodynamic barrier have hindered the realization of fast catalysis and bulk diffusion at low temperatures. Here, we report a significant lowering of the redox temperature by epitaxial stabilization of strontium cobaltites (SrCoOx) grown directly as one of two distinct crystalline phases, either the perovskite SrCoO3-delta or the brownmillerite SrCoO2.5. Importantly, these two phases can be reversibly switched at a remarkably reduced temperature (200-300 degrees C) in a considerably short time (<1 min) without destroying the parent framework. The fast, low-temperature redox activity in SrCoO3-delta is attributed to a small Gibbs free-energy difference between two topotatic phases. Our findings thus provide useful information for developing highly sensitive electrochemical sensors and low-temperature cathode materials. C1 [Jeen, Hyoungjeen; Choi, Woo Seok; Shin, Dongwon; Chisholm, Matthew F.; Lee, Ho Nyung] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Biegalski, Michael D.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Folkman, Chad M.; Fong, Dillon D.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Tung, I-Cheng; Freeland, John W.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Tung, I-Cheng] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. [Ohta, Hiromichi] Hokkaido Univ, Res Inst Elect Sci, Sapporo, Hokkaido 0010020, Japan. RP Lee, HN (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. EM hnlee@ornl.gov RI Choi, Woo Seok/G-8783-2014; Shin, Dongwon/C-6519-2008; Ohta, Hiromichi/H-4468-2012; Lee, Ho Nyung/K-2820-2012 OI Shin, Dongwon/0000-0002-5797-3423; Ohta, Hiromichi/0000-0001-7013-0343; Lee, Ho Nyung/0000-0002-2180-3975 FU US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division; Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy; US Department of Energy, Office of Science [DE-AC02-06CH11357]; MEXT [25246023] FX The work was supported by the US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. The in situ XRD measurement was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. Use of the Advanced Photon Source was supported by the US Department of Energy, Office of Science, under Contract No. DE-AC02-06CH11357. H.O. was supported by MEXT (25246023). NR 36 TC 68 Z9 68 U1 15 U2 113 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1476-1122 EI 1476-4660 J9 NAT MATER JI Nat. Mater. PD NOV PY 2013 VL 12 IS 11 BP 1057 EP 1063 DI 10.1038/NMAT3736 PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Materials Science; Physics GA 240LZ UT WOS:000326099300023 PM 23975056 ER PT J AU Thomas, JL AF Thomas, Jennifer L. TI Helpful or Harmful? Potential Effects of Exercise on Select Inflammatory Conditions SO PHYSICIAN AND SPORTSMEDICINE LA English DT Article DE inflammation; exercise; rheumatic diseases; cytokines; physical activity ID NECROSIS-FACTOR-ALPHA; NF-KAPPA-B; HUMAN SKELETAL-MUSCLE; UBIQUITIN-PROTEASOME PATHWAY; SYSTEMIC-LUPUS-ERYTHEMATOSUS; ANKYLOSING-SPONDYLITIS; INSULIN-RESISTANCE; RHEUMATOID-ARTHRITIS; ECCENTRIC EXERCISE; AEROBIC EXERCISE AB Inflammation has been characterized as a double-edged sword, requiring a balance between health as maintained by regular exercise and activities that would exacerbate inflammatory diseases. The influence of exercise on inflammation is complex and has been widely studied in both healthy patient populations as well as populations of patients with many inflammatory and/or autoimmune rheumatic diseases. Inflammatory markers can be affected by the type of exercise and muscle contraction, as well as the intensity, duration, and consistency of the exercise sessions. Because of these potentially important effects, many members of the general public, as well as some clinicians, believe that exercise could exacerbate symptoms and accelerate the progression of such conditions. The effects of different types of exercise have been studied among patients with inflammatory conditions such as ankylosing spondylitis, systemic lupus erythematosus, rheumatoid arthritis, osteoarthritis, fibromyalgia, and idiopathic inflammatory myopathies, as well as congestive heart failure, type 2 diabetes mellitus, and metabolic syndrome, which are considered lowgrade systemic inflammatory diseases. This review will help exercise professionals and clinicians understand the effects of exercise on inflammatory markers, as well as offer effective treatment options and recommendations for patients exercising with rheumatic or inflammatory conditions. C1 [Thomas, Jennifer L.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Thomas, Jennifer L.] Univ New Mexico, Dept Hlth Exercise & Sports Sci, Albuquerque, NM 87131 USA. RP Thomas, JL (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. NR 53 TC 6 Z9 6 U1 2 U2 15 PU JTE MULTIMEDIA PI WEST CONSHOHOCKEN PA 18 ELIZABETH ST, STE 110, WEST CONSHOHOCKEN, PA 19428 USA SN 0091-3847 J9 PHYSICIAN SPORTSMED JI Physician Sportsmed. PD NOV PY 2013 VL 41 IS 4 BP 93 EP 100 DI 10.3810/psm.2013.11.2040 PG 8 WC Primary Health Care; Orthopedics; Sport Sciences SC General & Internal Medicine; Orthopedics; Sport Sciences GA AR2FB UT WOS:000343397900010 PM 24231601 ER PT J AU Cornillon, PA Hengartner, N Jegou, N Matzner-Lober, E AF Cornillon, P-A Hengartner, N. Jegou, N. Matzner-Lober, E. TI Iterative bias reduction: a comparative study SO STATISTICS AND COMPUTING LA English DT Article DE Multivariate smoothing; Thin-plate splines; Duchon splines; Kernel regression; Iterative bias reduction ID GENERALIZED CROSS-VALIDATION; ADDITIVE LOGISTIC-REGRESSION; STATISTICAL VIEW; MODELS AB Multivariate nonparametric smoothers, such as kernel based smoothers and thin plate splines smoothers, are adversely impacted by the sparseness of data in high dimension, also known as the curse of dimensionality. Adaptive smoothers, that can exploit the underlying smoothness of the regression function, may partially mitigate this effect. This paper presents a comparative simulation study of a novel adaptive smoother (IBR) with competing multivariate smoothers available as package or function within the R language and environment for statistical computing. Comparison between the methods are made on simulated datasets of moderate size, from 50 to 200 observations, with two, five or 10 potential explanatory variables, and on a real dataset. The results show that the good asymptotic properties of IBR are complemented by a very good behavior on moderate sized datasets, results which are similar to those obtained with Duchon low rank splines. C1 [Cornillon, P-A] Univ Rennes 2, IRMAR, F-35043 Rennes, France. [Jegou, N.; Matzner-Lober, E.] Univ Rennes 2, F-35043 Rennes, France. [Hengartner, N.] Los Alamos Natl Lab, Los Alamos, NM USA. RP Matzner-Lober, E (reprint author), Univ Rennes 2, F-35043 Rennes, France. EM pac@uhb.fr; nickh@lanl.gov; nicolas.jegou@uhb.fr; eml@uhb.fr NR 32 TC 2 Z9 2 U1 1 U2 7 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0960-3174 J9 STAT COMPUT JI Stat. Comput. PD NOV PY 2013 VL 23 IS 6 BP 777 EP 791 DI 10.1007/s11222-012-9346-4 PG 15 WC Computer Science, Theory & Methods; Statistics & Probability SC Computer Science; Mathematics GA 214MS UT WOS:000324138300008 ER PT J AU Du, MH Biswas, K AF Du, Mao-Hua Biswas, Koushik TI Electronic structure engineering of elpasolites: Case of Cs2AgYCl6 SO JOURNAL OF LUMINESCENCE LA English DT Article DE Cs2AgYCl6; Elpasolite; Scintillator; Radiation detection ID DOPED HALIDE SCINTILLATORS; AUGMENTED-WAVE METHOD; ANOMALOUS EMISSION; CRYSTALS; GAMMA; CS2LIYCL6-CE3+; SPECTROSCOPY; EFFICIENT; GROWTH; RAY AB Electronic structure engineering of elpasolite-based scintillators is explored for improving light yield and scintillation response. First-principles calculations of electronic structure, polarons, and Ce activator in CS2AgYCl6 show that the electronegativity of constituent elements of a quaternary elpasolite compound can be manipulated to reduce the band gap and carrier self-trapping energy, which should lead to higher light yield and faster scintillation decay. (C) 2013 Elsevier B.V. All rights reserved. C1 [Du, Mao-Hua] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Du, Mao-Hua] Oak Ridge Natl Lab, Ctr Radiat Detect Mat & Syst, Oak Ridge, TN 37831 USA. [Biswas, Koushik] Arkansas State Univ, Dept Chem & Phys, State Univ, AR 72467 USA. RP Du, MH (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. EM mhdu@ornl.gov RI Du, Mao-Hua/B-2108-2010 OI Du, Mao-Hua/0000-0001-8796-167X FU U.S. Department of Energy's Office of Nonproliferation and Verification Research and Development [NA-22] FX We are grateful for helpful discussions with Zane W. Bell, David J. Singh and Lynn A. Boatner. This work was supported by the U.S. Department of Energy's Office of Nonproliferation and Verification Research and Development (NA-22). NR 32 TC 6 Z9 6 U1 2 U2 21 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-2313 J9 J LUMIN JI J. Lumines. PD NOV PY 2013 VL 143 BP 710 EP 714 DI 10.1016/j.jlumin.2013.05.033 PG 5 WC Optics SC Optics GA 211MN UT WOS:000323912400116 ER PT J AU Chou, CP AF Chou, Chung-Pin TI Low-lying quasiparticle excitations in strongly correlated superconductors: An ansatz from BCS quasiparticle excitations? SO JOURNAL OF PHYSICS AND CHEMISTRY OF SOLIDS LA English DT Article DE Superconductors; Variational Monte Carlo; Strong correlation; Quasiparticle excitations ID HIGH-TEMPERATURE SUPERCONDUCTIVITY; ANGLE-RESOLVED PHOTOEMISSION; MEAN-FIELD THEORY; FERMION SYSTEMS; MONTE-CARLO; SIMULATION AB The question about the existence of Bogoliubov's quasiparticles in the BCS wave functions underneath Gutzwiller's projection is of importance to strongly correlated systems. We develop a method to examine the two-particle excitations of Gutzwiller-projected BCS wave functions by using the variational Monte Carlo approach. We find that the exact Gutzwiller-projected quasiparticle (GQP) dispersions are quantitatively reproduced by the Gutzwiller-projected Bogoliubov quasiparticles (GBQP) except the regions where d-wave Cooper pairing is strong. We believe GBQP provides a reasonable description to the low-energy excitations in strongly correlated superconducting systems because GBQP becomes more stable than GQP near the antinodes. Our framework offers a route to understand the intimate connection between Gutzwiller's projection and d-wave Cooper pairing. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Chou, Chung-Pin] Beijing Computat Sci Res Ctr, Beijing 100084, Peoples R China. [Chou, Chung-Pin] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RP Chou, CP (reprint author), Beijing Computat Sci Res Ctr, Beijing 100084, Peoples R China. EM cpc63078@gmail.com FU Brookhaven Science Associates, LLC [DE-AC02-98CH10886]; U.S. Department of Energy; National Science Council in Taiwan [NSC 101-2917-I-564-010] FX The author thanks T.-K. Lee and W. Ku for useful discussions. We also acknowledge W. Yin for helpful proofreading on the manuscript. This work is supported by Brookhaven Science Associates, LLC under Contract no. DE-AC02-98CH10886 with the U.S. Department of Energy and the Postdoctoral Research Abroad Program sponsored by National Science Council in Taiwan with Grant no. NSC 101-2917-I-564-010. NR 36 TC 1 Z9 1 U1 0 U2 14 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0022-3697 J9 J PHYS CHEM SOLIDS JI J. Phys. Chem. Solids PD NOV PY 2013 VL 74 IS 11 BP 1589 EP 1593 DI 10.1016/j.jpcs.2013.05.027 PG 5 WC Chemistry, Multidisciplinary; Physics, Condensed Matter SC Chemistry; Physics GA 207HR UT WOS:000323590000012 ER PT J AU Lee, KJ Smith, K Pesaran, A Kim, GH AF Lee, Kyu-Jin Smith, Kandler Pesaran, Ahmad Kim, Gi-Heon TI Three dimensional thermal-, electrical-, and electrochemical-coupled model for cylindrical wound large format lithium-ion batteries SO JOURNAL OF POWER SOURCES LA English DT Article DE Lithium-ion battery; Wound cylindrical cell; Multiscale model; Orthotropic continuum; Wound potential-pair continuum model ID POSITIVE ELECTRODES; DESIGN; CELL AB A numerical model for cylindrical wound lithium-ion cells, which resolves thermal, electrical and electrochemical coupled physics, is presented in this paper. Using the Multi-Scale Multi-Domain (MSMD) model framework, the wound potential-pair continuum (WPPC) model is developed as a cell domain submodel to solve heat and electron transfer across the length scale of cell dimension. By defining the cell composite as a wound continuum, the WPPC model can evaluate layer-to-layer differences in electrical potential along current collectors, and electric current in the winding direction to investigate the effects of thermal and electrical configurations of a cell design, such as number and location of tabs, on performance and life of a cylindrical cell. In this study, 20-Ah large-format cylindrical cell simulations are conducted using the WPPC model with the number of electrical tabs as a control parameter to investigate how macroscopic design for electrical current transport affects microscopic electrochemical processes and apparent electrical and thermal output. (C) 2013 Elsevier B.V. All rights reserved. C1 [Lee, Kyu-Jin; Smith, Kandler; Pesaran, Ahmad; Kim, Gi-Heon] Natl Renewable Energy Lab, Golden, CO USA. [Lee, Kyu-Jin] Myongji Univ, Dept Mech Engn, Yongin, Gyeonggi Do, South Korea. RP Kim, GH (reprint author), Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO USA. EM gi-heon.kim@nrel.gov RI Khan, Mohammad Rezwan/E-1422-2011 OI Khan, Mohammad Rezwan/0000-0002-1532-0598 FU U.S. Department of Energy Office of Vehicle Technologies' Energy Storage Program; U.S. DOE's Computer Aided Engineering for Electric Drive Batteries (CAEBat) FX The authors acknowledge David Howell, Brian Cunningham, and the U.S. Department of Energy Office of Vehicle Technologies' Energy Storage Program for their funding and support. The present work was supported by the U.S. DOE's Computer Aided Engineering for Electric Drive Batteries (CAEBat). NR 21 TC 39 Z9 40 U1 5 U2 74 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 J9 J POWER SOURCES JI J. Power Sources PD NOV 1 PY 2013 VL 241 BP 20 EP 32 DI 10.1016/j.jpowsour.2013.03.007 PG 13 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA 200TL UT WOS:000323093700004 ER PT J AU Vijayakumar, M Wang, W Nie, ZM Sprenkle, V Hu, JZ AF Vijayakumar, M. Wang, Wei Nie, Zimin Sprenkle, Vincent Hu, JianZhi TI Elucidating the higher stability of vanadium(V) cations in mixed acid based redox flow battery electrolytes SO JOURNAL OF POWER SOURCES LA English DT Article DE Cl-35 and V-51 NMR; Vanadium redox flow battery; Electrolyte stability and DFT; Ligand exchange process ID RESEARCH-AND-DEVELOPMENT; ENERGY-STORAGE; DENSITY; PROGRESS; CELL; THERMOCHEMISTRY; APPROXIMATION; ORBITALS AB The vanadium(V) cation structures in mixed acid based electrolyte solution were analyzed by density functional theory (DFT) based computational modeling and V-51 and Cl-35 nuclear magnetic resonance (NMR) spectroscopy. The vanadium(V) cation exists as di-nuclear [V2O3Cl2 center dot 6H(2)O](2+) compound at higher vanadium concentrations (>= 1.75 M). In particular, at high temperatures (>295 K) this di-nuclear compound undergoes ligand exchange process with nearby solvent chlorine molecule and forms chlorine bonded [V2O3Cl center dot 6H(2)O](2+) compound. This chlorine bonded [V2O3Cl2 center dot 6H(2)O]2+ compound might be resistant to the de-protonation reaction which is the initial step in the precipitation reaction in vanadium based electrolyte solutions. The combined theoretical and experimental approach reveals that formation of chlorine bonded [V2O3Cl2 center dot 6H(2)O](2+) compound might be central to the observed higher thermal stability of mixed acid based vanadium(V) electrolyte solutions. (C) 2013 Elsevier B.V. All rights reserved. C1 [Vijayakumar, M.; Wang, Wei; Nie, Zimin; Sprenkle, Vincent; Hu, JianZhi] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Vijayakumar, M (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM Vijay@pnnl.gov; wei.wang@pnnl.gov RI Murugesan, Vijayakumar/C-6643-2011; Wang, Wei/F-4196-2010; Hu, Jian Zhi/F-7126-2012 OI Murugesan, Vijayakumar/0000-0001-6149-1702; Wang, Wei/0000-0002-5453-4695; FU Office of Electricity Delivery & Energy Reliability; U.S. Department of Energy (DOE) [57558]; PNNL through LDRD program; DOE by Battelle [DE-AC05-76RL01830]; DOE's Office of Biological and Environmental Research (BER) FX This work was supported by the Office of Electricity Delivery & Energy Reliability (project manager: Dr. Imre Gyuk), U.S. Department of Energy (DOE) under contract #57558. We also are grateful for insightful discussions with Dr. Imre Gyuk of the DOE-OE Grid Storage Program. We also acknowledge PNNL for the funding through LDRD program. PNNL is a multi-program laboratory operated for DOE by Battelle under Contract DE-AC05-76RL01830. The NMR and DFT computation work were carried out at the Environmental and Molecular Science Laboratory (EMSL), a national scientific user facility sponsored by the DOE's Office of Biological and Environmental Research (BER). We thank Sarah D. Burton from EMSL for her help in measuring NMR. NR 27 TC 25 Z9 26 U1 1 U2 104 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD NOV 1 PY 2013 VL 241 BP 173 EP 177 DI 10.1016/j.jpowsour.2013.04.072 PG 5 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA 200TL UT WOS:000323093700021 ER PT J AU Kalnaus, S Tenhaeff, WE Sakamoto, J Sabau, AS Daniel, C Dudney, NJ AF Kalnaus, Sergiy Tenhaeff, Wyatt E. Sakamoto, Jeffrey Sabau, Adrian S. Daniel, Claus Dudney, Nancy J. TI Analysis of composite electrolytes with sintered reinforcement structure for energy storage applications SO JOURNAL OF POWER SOURCES LA English DT Article DE Lithium ion battery; Composite electrolyte; Sintering; Lithium anode; Dendrites ID LITHIUM SECONDARY BATTERIES; SOLID POLYMER ELECTROLYTES; THIN-FILM LITHIUM; ELASTIC PROPERTIES; ION BATTERIES; ELECTRICAL-PROPERTIES; GLASS-CERAMICS; CONDUCTIVITY; MODULUS; LI7LA3ZR2O12 AB Effective conductivity and mechanical properties of composite polymer electrolytes, in which the reinforcement phase is a sintered packed bed of Li-ion conductive ceramics particles, were estimated using finite element analyses. The computations targeted estimation of the effect of sintering degree, i.e. size of the inter-particle connective necks, on the overall properties of the composite. Methods for microstructure generation and computational procedures were presented. The mechanical ability of the membrane to block lithium dendrites was assessed based on a stability criterion, which depends on the computed effective stiffness. It was found that the minimum size of the inter-particle connections necessary to provide mechanical stability without losing the enhancement in conductivity was 0.05 times the mean particle radius. (C) 2013 Elsevier B.V. All rights reserved. C1 [Kalnaus, Sergiy; Tenhaeff, Wyatt E.; Sabau, Adrian S.; Daniel, Claus; Dudney, Nancy J.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Sakamoto, Jeffrey] Michigan State Univ, Dept Mat Sci & Engn, E Lansing, MI 48824 USA. [Daniel, Claus] Oak Ridge Natl Lab, Energy & Transportat Sci Div, Oak Ridge, TN 37831 USA. [Daniel, Claus] Univ Tennessee, Bredesen Ctr Interdisciplinary Res & Grad Educ, Knoxville, TN 37996 USA. RP Kalnaus, S (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. EM kalnauss@oml.gov RI Sabau, Adrian/B-9571-2008; Dudney, Nancy/I-6361-2016; Daniel, Claus/A-2060-2008; OI Sabau, Adrian/0000-0003-3088-6474; Dudney, Nancy/0000-0001-7729-6178; Daniel, Claus/0000-0002-0571-6054; Kalnaus, Sergiy/0000-0002-7465-3034 FU U.S. Department of Energy [DE-AC05-00OR22725]; Vehicle Technologies Program for the Office of Energy Efficiency and Renewable Energy; Laboratory Directed Research and Development Program (LDRD) of ORNL; Office of Naval Research FX This research at Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy under contract DE-AC05-00OR22725, was sponsored by the Vehicle Technologies Program for the Office of Energy Efficiency and Renewable Energy. The seeding algorithm was developed in earlier work sponsored by the Laboratory Directed Research and Development Program (LDRD) of ORNL. Work at Michigan State University was supported by the Office of Naval Research. NR 42 TC 2 Z9 2 U1 2 U2 105 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 J9 J POWER SOURCES JI J. Power Sources PD NOV 1 PY 2013 VL 241 BP 178 EP 185 DI 10.1016/j.jpowsour.2013.04.096 PG 8 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA 200TL UT WOS:000323093700022 ER PT J AU Suss, ME Baumann, TF Worsley, MA Rose, KA Jaramillo, TF Stadermann, M Santiago, JG AF Suss, Matthew E. Baumann, Theodore F. Worsley, Marcus A. Rose, Klint A. Jaramillo, Thomas F. Stadermann, Michael Santiago, Juan G. TI Impedance-based study of capacitive porous carbon electrodes with hierarchical and bimodal porosity SO JOURNAL OF POWER SOURCES LA English DT Article DE Energy storage; Carbon aerogel; Supercapacitor; Capacitive deionization; Electrochemical impedance spectroscopy; Hierarchical carbon ID ELECTROCHEMICAL CAPACITORS; CONCENTRATION POLARIZATION; RATE CAPABILITY; WATER; SUPERCAPACITORS; DESALINATION; DEIONIZATION; SPECTROSCOPY; PROPAGATION; ENERGY AB Porous electrode capacitors are used extensively in systems which store energy, harvest mixing energy, or desalinate water. These electrodes can possess a hierarchical pore structure with larger macroscale pores allowing for facile ion and fluid transport, and smaller, nanometer-scale pores enabling significant ion storage. We here present a combined theoretical (linear circuit model) and experimental (electrochemical impedance spectroscopy) study of porous carbon electrode capacitors which integrate nanoscale pores into a micron-scale porous network. Our experiments are performed on a set of custom-fabricated hierarchical carbon aerogel electrodes with varying pore structure, including electrodes with sub-nanometer (sub-nm) pores. Our combined theory and experimental approach allows us to demonstrate the utility of our model, perform detailed characterizations of our electrodes, study the effects of pore structure variations on impedance, and propose hierarchical electrode design and characterization guidelines. Further, we demonstrate that our approach is promising toward the detailed study of ion storage mechanisms in sub-nm pores. (C) 2013 Elsevier B.V. All rights reserved. C1 [Suss, Matthew E.; Santiago, Juan G.] Stanford Univ, Dept Mech Engn, Stanford, CA 94305 USA. [Suss, Matthew E.; Baumann, Theodore F.; Worsley, Marcus A.; Rose, Klint A.; Stadermann, Michael] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Jaramillo, Thomas F.] Stanford Univ, Dept Chem Engn, Stanford, CA 94305 USA. RP Stadermann, M (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. EM stadermann2@llnl.gov; juan.santiago@stanford.edu RI Jaramillo, Thomas/C-4174-2014; Worsley, Marcus/G-2382-2014 OI Jaramillo, Thomas/0000-0001-9900-0622; Worsley, Marcus/0000-0002-8012-7727 FU National Science Foundation [0967600]; State of California's Proposition 50 funds; Natural Sciences and Engineering Research Council (NSERC) of Canada; US DOE by LLNL [DE-AC52-07NA27344] FX This work was supported by the National Science Foundation under grant no. 0967600 and State of California's Proposition 50 funds administered by the Department of Water Resources. Any opinions, findings, and conclusions or recommendations expressed in this material are those of the authors and do not necessarily reflect the views of the National Science Foundation. MES would like to thank the Lawrence Scholar program and a postgraduate scholarship from the Natural Sciences and Engineering Research Council (NSERC) of Canada. Work at LLNL was performed under the auspices of the US DOE by LLNL under Contract DE-AC52-07NA27344. We would like to thank Kendra Kuhl, Benjamin Reinecke, Zhebo Chen, and Etosha Cave for their training and technical assistance in the use of three-electrode cells and the potentiostat. NR 42 TC 21 Z9 21 U1 8 U2 185 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD NOV 1 PY 2013 VL 241 BP 266 EP 273 DI 10.1016/j.jpowsour.2013.03.178 PG 8 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA 200TL UT WOS:000323093700034 ER PT J AU He, QP Joy, DC Keffer, DJ AF He, Qianping Joy, David C. Keffer, David J. TI Nanoparticle adhesion in proton exchange membrane fuel cell electrodes SO JOURNAL OF POWER SOURCES LA English DT Article DE Nanoparticle adhesion; PEM fuel cell; Carbon supported platinum catalyst; Catalyst deactivation; Nafion ID MOLECULAR-DYNAMICS SIMULATION; DOPED CARBON NANOTUBES; SURFACE-AREA LOSS; PHOSPHORIC-ACID; PLATINUM NANOPARTICLES; CATALYST DEGRADATION; NAFION; DURABILITY; ELECTROCATALYSTS; WATER AB Carbon supported platinum (Pt/C) catalyst remains among the most preferable catalyst materials for Proton Exchange Membrane (PEM) fuel cells. However, platinum (Pt) particles suffer from poor durability and encounter electrochemical surface area (ESA) loss under operation with the accompany of Pt nanoparticle coarsening. Several proposed mechanisms have involved the Pt detachment from its carbonate support as an initial step for the deactivation of Pt nanoparticles. In this study, we investigated the detachment mechanism from the nano-adhesion point of view. Classic molecular dynamics simulations are performed on systems contain Pt nanoparticles of different sizes and shapes. A thin Nafion film (1 nm) at different hydration levels is also included in the system to study the environmental effect on nanoparticle adhesion. We found that the adhesion force strengthens as the Pt size goes up. Pt nanoparticles of tetrahedral shape exhibit relatively stronger connection with the carbon substrate due to its unique 'anchor-like' structure. Adhesion is enhanced with the introduction of a Nafion. The humidity level in the Nafion film has a rather complicated effect on the strength of nanoparticle adhesion. The binding energies and maximum adhesive forces are reported for all systems studied. (C) 2013 Elsevier B.V. All rights reserved. C1 [He, Qianping] Univ Tennessee, Dept Chem & Biomol Engn, Knoxville, TN 37996 USA. [Joy, David C.; Keffer, David J.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Joy, David C.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37830 USA. RP Keffer, DJ (reprint author), Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. EM dkeffer@utk.edu RI Keffer, David/C-5133-2014 OI Keffer, David/0000-0002-6246-0286 FU Sustainable Energy and Education Research Center at the University of Tennessee; National Science Foundation [DGE-0801470]; US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; NSF [OCI 07-11134.5] FX This research was supported by the Sustainable Energy and Education Research Center at the University of Tennessee, by a grant from the National Science Foundation (DGE-0801470) and by the US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. This research project used resources of the National Institute for Computational Sciences (NICS) supported by NSF under agreement number: OCI 07-11134.5. NR 79 TC 11 Z9 13 U1 6 U2 100 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 J9 J POWER SOURCES JI J. Power Sources PD NOV 1 PY 2013 VL 241 BP 634 EP 646 DI 10.1016/j.jpowsour.2013.05.011 PG 13 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA 200TL UT WOS:000323093700082 ER PT J AU Zerovnik, G Trkov, A Smith, DL Capote, R AF Zerovnik, Gasper Trkov, Andrej Smith, Donald L. Capote, Roberto TI Transformation of correlation coefficients between normal and lognormal distribution and implications for nuclear applications SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Multivariate normal distribution; Multivariate lognormal distribution; Correlation matrix; Evaluated nuclear data formats ID UNIFIED MONTE-CARLO AB Inherently positive parameters with large relative uncertainties (typically greater than or similar to 300) are often considered to be governed by the lognormal distribution. This assumption has the practical benefit of avoiding the possibility of sampling negative values in stochastic applications. Furthermore, it is typically assumed that the correlation coefficients for comparable multivariate normal and lognormal distributions are equivalent. However, this ideal situation is approached only in the linear approximation which happens to be applicable just for small uncertainties. This paper derives and discusses the proper transformation of correlation coefficients between both distributions for the most general case which is applicable for arbitrary uncertainties. It is seen that for lognormal distributions with large relative uncertainties strong anti-correlations (negative correlations) are mathematically forbidden. This is due to the asymmetry that is an inherent feature of these distributions. Some implications of these results for practical nuclear applications are discussed and they are illustrated with examples in this paper. Finally, modifications to the ENDF-6 format used for representing uncertainties in evaluated nuclear data libraries are suggested, as needed to deal with this issue. (C) 2013 Elsevier B.V. All rights reserved. C1 [Zerovnik, Gasper; Trkov, Andrej] Jozef Stefan Inst, SI-1000 Ljubljana, Slovenia. [Smith, Donald L.] Argonne Natl Lab, Coronado, CA 92118 USA. [Capote, Roberto] IAEA, NAPC Nucl Data Sect, A-1400 Vienna, Austria. RP Zerovnik, G (reprint author), Jozef Stefan Inst, Jamova Cesta 39, SI-1000 Ljubljana, Slovenia. EM gasper.zerovnik@ijs.si; andrej.trkov@ijs.si; donald.l.smith@anl.gov; roberto.capotenoy@iaea.org RI Capote Noy, Roberto/M-1245-2014 OI Capote Noy, Roberto/0000-0002-1799-3438 NR 11 TC 8 Z9 8 U1 0 U2 8 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD NOV 1 PY 2013 VL 727 BP 33 EP 39 DI 10.1016/j.nima.2013.06.025 PG 7 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 206WY UT WOS:000323557700006 ER PT J AU Best, A Couder, M Famiano, M Lemut, A Wiescher, M AF Best, Andreas Couder, Manoel Famiano, Michael Lemut, Alberto Wiescher, Michael TI Study of the beam-induced neutron flux and required shielding for DIANA SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Neutron shielding; Monte Carlo simulation; Underground laboratory ID GEANT4 AB Low energy accelerators in underground locations have emerged as a powerful tool for the measurement of critical nuclear reactions for the study of energy production and element synthesis in astrophysics. While cosmic ray induced background is substantially reduced, beam induced background on target impurities and depositions on target and collimator materials remain a matter of serious concern. The Dual Ion Accelerator for Nuclear Astrophysics (DIANA) is proposed to operate as a low-level background facility in an underground location. One of the main goals of DIANA is the study of neutron sources in stellar helium burning. For these experiments DIANA is a neutron radiation source which may affect other nearby low background level experiments. We therefore investigated the required laboratory layout to attenuate the neutron flux generated in a worst-case scenario to a level below the natural background in the underground environment. Detailed Monte Carlo calculations of the neutron propagation in the laboratory show that a neutron flux many orders of magnitude above expected values gets attenuated below the natural background rate using a 1 m thick water-shielded door as well as an emergency access/egress maze. (C) 2013 Elsevier B.V. All rights reserved. C1 [Best, Andreas; Couder, Manoel; Wiescher, Michael] Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. [Best, Andreas; Couder, Manoel; Wiescher, Michael] Univ Notre Dame, Joint Inst Nucl Astrophys, Notre Dame, IN 46556 USA. [Best, Andreas; Lemut, Alberto] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Famiano, Michael] Western Michigan Univ, Dept Phys, Kalamazoo, MI 49008 USA. RP Best, A (reprint author), Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. EM abest1@nd.edu RI Couder, Manoel/B-1439-2009; OI Couder, Manoel/0000-0002-0636-744X; Best, Andreas/0000-0001-8869-9757 FU National Science Foundation [PHY-0918728]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Building Technology, State, and Community Programs, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the National Science Foundation through Grant number PHY-0918728. This work was also supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract no. DE-AC02-05CH11231 and by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Building Technology, State, and Community Programs, of the U.S. Department of Energy under Contract no. DE-AC02-05CH11231. NR 28 TC 5 Z9 5 U1 0 U2 29 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD NOV 1 PY 2013 VL 727 BP 104 EP 108 DI 10.1016/j.nima.2013.06.032 PG 5 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 206WY UT WOS:000323557700016 ER PT J AU Gidalevitz, T Stevens, F Argon, Y AF Gidalevitz, Tali Stevens, Fred Argon, Yair TI Orchestration of secretory protein folding by ER chaperones SO BIOCHIMICA ET BIOPHYSICA ACTA-MOLECULAR CELL RESEARCH LA English DT Review DE Endoplasmic reticulum; Chaperones; Protein folding; Secretome ID ENDOPLASMIC-RETICULUM CHAPERONES; DISULFIDE BOND FORMATION; VIRUS-G PROTEIN; MHC CLASS-I; PHOSPHATIDYLSERINE-CONTAINING MEMBRANES; NEMATODE CAENORHABDITIS-ELEGANS; HUMAN CHORIONIC-GONADOTROPIN; NUCLEOTIDE EXCHANGE FACTOR; MARINESCO-SJOGREN-SYNDROME; NEWLY SYNTHESIZED PROTEINS AB The endoplasmic reticulum is a major compartment of protein biogenesis in the cell, dedicated to production of secretory, membrane and organelle proteins. The secretome has distinct structural and post-translational characteristics, since folding in the ER occurs in an environment that is distinct in terms of its ionic composition, dynamics and requirements for quality control. The folding machinery in the ER therefore includes chaperones and folding enzymes that introduce, monitor and react to disulfide bonds, glycans, and fluctuations of luminal calcium. We describe the major chaperone networks in the lumen and discuss how they have distinct modes of operation that enable cells to accomplish highly efficient production of the secretome. This article is part of a Special Issue entitled: Functional and structural diversity of endoplasmic reticulum. (c) 2013 Elsevier B.V. All rights reserved. C1 [Gidalevitz, Tali] Drexel Univ, Dept Biol, Philadelphia, PA 19104 USA. [Stevens, Fred] Argonne Natl Lab, Argonne, IL 60439 USA. [Argon, Yair] Childrens Hosp Philadelphia, Dept Pathol & Lab Med, Div Cell Pathol, Philadelphia, PA 19104 USA. [Argon, Yair] Univ Penn, Philadelphia, PA 19104 USA. RP Argon, Y (reprint author), Childrens Hosp Philadelphia, Dept Pathol & Lab Med, Div Cell Pathol, 3615 Civ Ctr Blvd, Philadelphia, PA 19104 USA. EM yargon@mail.med.upenn.edu RI Gidalevitz, Tali/C-9217-2009 FU NIH [AG18001, GM07748] FX We thank Drs. J. Brodsky (Univ. Pitt.), E. Snapp (Albert Einstein College of Medicine), M. Molinari (Institute for Research in Biomedicine, Bellinzona, Switserland), P. Cresswell (Yale Univ.) and D. Hebert (Univ. Mass.) for helpful comments and personal communications. Work in the authors' lab was supported by NIH grants AG18001 and GM07748. NR 241 TC 37 Z9 39 U1 3 U2 60 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-4889 EI 0006-3002 J9 BBA-MOL CELL RES JI Biochim. Biophys. Acta-Mol. Cell Res. PD NOV PY 2013 VL 1833 IS 11 SI SI BP 2410 EP 2424 DI 10.1016/j.bbamcr.2013.03.007 PG 15 WC Biochemistry & Molecular Biology; Cell Biology SC Biochemistry & Molecular Biology; Cell Biology GA 204VS UT WOS:000323400000004 PM 23507200 ER PT J AU Givens, GH Beveridge, JR Phillips, PJ Draper, B Lui, YM Bolme, D AF Givens, G. H. Beveridge, J. R. Phillips, P. J. Draper, B. Lui, Y. M. Bolme, D. TI Introduction to face recognition and evaluation of algorithm performance SO COMPUTATIONAL STATISTICS & DATA ANALYSIS LA English DT Article DE Face recognition; Biometrics; Computer vision; Generalized linear mixed model; GLMM ID LINEAR MIXED MODELS; GRAND CHALLENGE; DISCRIMINANT-ANALYSIS; LIKELIHOOD; INFERENCE; FEATURES; IMAGES; SYSTEM AB The field of biometric face recognition blends methods from computer science, engineering and statistics, however statistical reasoning has been applied predominantly in the design of recognition algorithms. A new opportunity for the application of statistical methods is driven by growing interest in biometric performance evaluation. Methods for performance evaluation seek to identify, compare and interpret how characteristics of subjects, the environment and images are associated with the performance of recognition algorithms. Some central topics in face recognition are reviewed for background and several examples of recognition algorithms are given. One approach to the evaluation problem is then illustrated with a generalized linear mixed model analysis of the Good, Bad, and Ugly Face Challenge, a pre-eminent face recognition dataset used to test state-of-the-art still-image face recognition algorithms. Findings include that (i) between-subject variation is the dominant source of verification heterogeneity when algorithm performance is good, and (ii) many covariate effects on verification performance are 'universal' across easy, medium and hard verification tasks. Although the design and evaluation of face recognition algorithms draw upon some familiar statistical ideas in multivariate statistics, dimension reduction, classification, clustering, binary response data, generalized linear models and random effects, the field also presents some unique features and challenges. Opportunities abound for innovative statistical work in this new field. (C) 2013 Elsevier B.V. All rights reserved. C1 [Givens, G. H.] Colorado State Univ, Dept Stat, Ft Collins, CO 80523 USA. [Beveridge, J. R.; Draper, B.; Lui, Y. M.] Colorado State Univ, Dept Comp Sci, Ft Collins, CO 80523 USA. [Phillips, P. J.] NIST, Gaithersburg, MD 20899 USA. [Bolme, D.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Givens, GH (reprint author), Colorado State Univ, Dept Stat, Ft Collins, CO 80523 USA. EM geof@lamar.colostate.edu FU Technical Support Working Group (TSWG) [SC-AS-3181C]; Federal Bureau of Investigation (FBI) FX This work was supported by the Technical Support Working Group (TSWG) under Task SC-AS-3181C. P. Jonathon Phillips thanks the Federal Bureau of Investigation (FBI) for their support of this work. The identification of any commercial product or trade name does not imply endorsement or recommendation by Colorado State University and the National Institute of Standards. NR 46 TC 12 Z9 13 U1 0 U2 57 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-9473 J9 COMPUT STAT DATA AN JI Comput. Stat. Data Anal. PD NOV PY 2013 VL 67 BP 236 EP 247 DI 10.1016/j.csda.2013.05.025 PG 12 WC Computer Science, Interdisciplinary Applications; Statistics & Probability SC Computer Science; Mathematics GA 203MJ UT WOS:000323297000018 ER PT J AU Wu, X Baker, I Miller, MK More, KL Cai, Z Chen, S AF Wu, X. Baker, I. Miller, M. K. More, K. L. Cai, Z. Chen, S. TI Microstructure and mechanical properties of two-phase Fe30Ni20Mn20Al30. Part I: Microstructure SO JOURNAL OF MATERIALS SCIENCE LA English DT Article ID LONG-RANGE ORDER; COMPOSITION DEPENDENCE; MODULATED STRUCTURE; YOUNG MODULUS; ALLOY; TEMPERATURE; PRECIPITATION; STRENGTH; PHASE; FE35NI15MN25AL25 AB The microstructure of Fe30Ni20Mn20Al30 in both the as-cast condition and after annealing at 823 K for various times up to 72 h was characterized using transmission electron microscopy, scanning transmission electron microscopy, synchrotron-based X-ray diffraction, and atom probe tomography. The microstructure exhibited a basketweave morphology of (Mn, Fe)-rich B2-ordered (ordered b.c.c.) and (Ni, Al)-rich L2(1)-ordered (Heusler type) phases with a lattice misfit of only 0.85 % and interfaces aligned along aOE (c) 100 >. The phase width increased from 5 nm for the as-cast alloy to 25 nm for 72 h annealed material, with no change in the elemental partitioning between the phases, with a time exponent for the coarsening kinetics of 0.19. Surprisingly, it was found that the room temperature hardness was largely independent of the phase width. C1 [Wu, X.; Baker, I.] Dartmouth Coll, Thayer Sch Engn, Hanover, NH 03755 USA. [Miller, M. K.; More, K. L.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Cai, Z.; Chen, S.] Argonne Natl Lab, Adv Photon Source, X Ray Sci Div, Argonne, IL 60439 USA. RP Baker, I (reprint author), Dartmouth Coll, Thayer Sch Engn, Hanover, NH 03755 USA. EM ian.baker@dartmouth.edu RI More, Karren/A-8097-2016 OI More, Karren/0000-0001-5223-9097 FU US Department of Energy (DOE), Office of Basic Energy Sciences [DE-FG02-07ER46392]; ORNL's ShaRE User Facility; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; U.S. DOE [DE-AC02-06CH11357] FX This research was supported by the US Department of Energy (DOE), Office of Basic Energy Sciences grant DE-FG02-07ER46392 (X. W and I. B). Research was supported ORNL's ShaRE User Facility, which is sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy (M. K. M. and K. L. M.). Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357 (Z. C. and S. C.). The authors gratefully acknowledge K. F. Russell for technical assistance. Prof. Paul Munroe of the University of New South Wales is thanked for the electron probe microanalyzer measurements. We would also like to thanks the reviewers for their numerous useful comments. The views and conclusions contained herein are those of the authors and should not be interpreted as necessarily representing official policies, either expressed or implied of the DOE or the U.S. Government. NR 46 TC 2 Z9 2 U1 0 U2 24 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0022-2461 EI 1573-4803 J9 J MATER SCI JI J. Mater. Sci. PD NOV PY 2013 VL 48 IS 21 BP 7435 EP 7445 DI 10.1007/s10853-013-7558-4 PG 11 WC Materials Science, Multidisciplinary SC Materials Science GA 202VW UT WOS:000323249500010 ER PT J AU Pilania, G Sharma, V AF Pilania, G. Sharma, Vinit TI First principles investigations of structural, electronic, elastic, and dielectric properties of KMgF3 SO JOURNAL OF MATERIALS SCIENCE LA English DT Article ID GENERALIZED GRADIENT APPROXIMATION; FUNCTIONAL PERTURBATION-THEORY; AB-INITIO; PEROVSKITE OXIDES; FORCE-CONSTANTS; DOPED KMGF3; CRYSTAL; IMPURITIES; PRESSURE; FLUORIDE AB An ab initio study of structural, electronic, elastic, and dielectric properties of KMgF3 in cubic perovskite structure is presented in the framework of density functional theory. The calculations presented here employ generalized gradient approximation with projector augmented wave method. The fully relaxed structural parameters are found to be in reasonable agreement with available experimental data and with previous theoretical work. The independent elastic constants of cubic KMgF3 are derived from the derivative of total energy as a function of lattice strain in full detail. The bulk modulus and its first pressure derivative are obtained by fitting total energy versus volume data to a Murnaghan equation of state. The electronic band structure, total density of states, and projected density of states on each of the K, Mg, and F atoms are calculated and found to be in good agreement with previous theoretical results. First principles computed phonon dispersions for the cubic KMgF3 are reported for the first time. The imaginary part of frequency-dependent dielectric function is determined by summing over all possible transitions from occupied to unoccupied states and taking the appropriate transition matrix element into account. The Born effective charges computed by linear response within density functional perturbation theory are used together with the mode eigenvectors to decompose the lattice dielectric susceptibility tensor into contributions arising from individual IR-active phonon modes. Our results for the static and optical dielectric constant are in good agreement with previously reported experimental results. C1 [Pilania, G.] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. [Sharma, Vinit] Univ Connecticut, Storrs, CT 06269 USA. RP Pilania, G (reprint author), Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. EM gpilania@gmail.com RI Pilania, Ghanshyam/K-4468-2013; sharma, Vinit/K-3407-2015 OI Pilania, Ghanshyam/0000-0003-4460-1572; NR 46 TC 3 Z9 3 U1 3 U2 35 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0022-2461 EI 1573-4803 J9 J MATER SCI JI J. Mater. Sci. PD NOV PY 2013 VL 48 IS 21 BP 7635 EP 7641 DI 10.1007/s10853-013-7581-5 PG 7 WC Materials Science, Multidisciplinary SC Materials Science GA 202VW UT WOS:000323249500033 ER PT J AU Romano, PK Siegel, AR Forget, B Smith, K AF Romano, Paul K. Siegel, Andrew R. Forget, Benoit Smith, Kord TI Data decomposition of Monte Carlo particle transport simulations via tally servers SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Monte Carlo; Neutron transport; Data decomposition; Exascale; Tally server ID ALGORITHMS AB An algorithm for decomposing large tally data in Monte Carlo particle transport simulations is developed, analyzed, and implemented in a continuous-energy Monte Carlo code, OpenMC. The algorithm is based on a non-overlapping decomposition of compute nodes into tracking processors and tally servers. The former are used to simulate the movement of particles through the domain while the latter continuously receive and update tally data. A performance model for this approach is developed, suggesting that, for a range of parameters relevant to LWR analysis, the tally server algorithm should perform with minimal overhead on contemporary supercomputers. An implementation of the algorithm in OpenMC is then tested on the Intrepid and Titan supercomputers, supporting the key predictions of the model over a wide range of parameters. We thus conclude that the tally server algorithm is a successful approach to circumventing classical on-node memory constraints en route to unprecedentedly detailed Monte Carlo reactor simulations. (C) 2013 Elsevier Inc. All rights reserved. C1 [Romano, Paul K.; Forget, Benoit; Smith, Kord] MIT, Dept Nucl Sci & Engn, Cambridge, MA 02139 USA. [Siegel, Andrew R.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Romano, PK (reprint author), MIT, Dept Nucl Sci & Engn, 77 Massachusetts Ave, Cambridge, MA 02139 USA. EM paul.k.romano@gmail.com; siegala@mcs.anl.gov; bforget@mit.edu; kord@mit.edu OI Romano, Paul/0000-0002-1147-045X FU Naval Reactors Division of the U.S Department of Energy; Office of Advanced Scientific Computing Research, Office of Science, US Department of Energy [DE-AC02-06CH11357]; Consortium for Advanced Simulation of Light Water Reactors, an Energy Innovation Hub for Modeling and Simulation of Nuclear Reactors under US Department of Energy [DE-AC05-00OR22725] FX This research was performed under appointment of the first author to the Rickover Fellowship Program in Nuclear Engineering sponsored by Naval Reactors Division of the U.S Department of Energy. This work was also supported in part by the Office of Advanced Scientific Computing Research, Office of Science, US Department of Energy, under Contract DE-AC02-06CH11357 and by the Consortium for Advanced Simulation of Light Water Reactors, an Energy Innovation Hub for Modeling and Simulation of Nuclear Reactors under US Department of Energy Contract No. DE-AC05-00OR22725. The authors would also like to thank Forrest Brown for advice and guidance regarding data decomposition. NR 17 TC 8 Z9 9 U1 1 U2 18 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 J9 J COMPUT PHYS JI J. Comput. Phys. PD NOV 1 PY 2013 VL 252 BP 20 EP 36 DI 10.1016/j.jcp.2013.06.011 PG 17 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA 194KZ UT WOS:000322633500002 ER PT J AU Scovazzi, G Huang, H Collis, SS Yin, J AF Scovazzi, G. Huang, H. Collis, S. S. Yin, J. TI A fully-coupled upwind discontinuous Galerkin method for incompressible porous media flows: High-order computations of viscous fingering instabilities in complex geometry SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Viscous fingering; Discontinuous Galerkin method; Porous media flows ID MISCIBLE DISPLACEMENT PROBLEMS; QUARTER 5-SPOT CONFIGURATION; REACTIVE TRANSPORT PROBLEMS; LINEAR-STABILITY ANALYSIS; IMMISCIBLE 2-PHASE FLOW; FINITE-ELEMENT METHODS; ELLIPTIC PROBLEMS; PERMEABILITY HETEROGENEITY; NUMERICAL-SIMULATION; DARCY FLOW AB We present a new approach to the simulation of viscous fingering instabilities in incompressible, miscible displacement flows in porous media. In the past, high resolution computational simulations of viscous fingering instabilities have always been performed using high-order finite difference or Fourier-spectral methods which do not posses the flexibility to compute very complex subsurface geometries. Our approach, instead, by means of a fully-coupled nonlinear implementation of the discontinuous Galerkin method, possesses a fundamental differentiating feature, in that it maintains high-order accuracy on fully unstructured meshes. In addition, the proposed method shows very low sensitivity to mesh orientation, in contrast with classical finite volume approximation used in porous media flow simulations. The robustness and accuracy of the method are demonstrated in a number of challenging computational problems. (C) 2013 Elsevier Inc. All rights reserved. C1 [Scovazzi, G.] Duke Univ, Dept Civil & Environm Engn, Durham, NC 27708 USA. [Huang, H.; Yin, J.] ExxonMobil Upstream Res Co, Houston, TX 77252 USA. [Collis, S. S.] Sandia Natl Labs, Numer Anal & Applicat Dept, Albuquerque, NM 87185 USA. RP Scovazzi, G (reprint author), Duke Univ, Dept Civil & Environm Engn, Room 121,Hudson Hall,POB 90287, Durham, NC 27708 USA. EM guglielmo.scovazzi@duke.edu RI Huang, Hao/A-1376-2012; OI Huang, Hao/0000-0002-5186-180X; Yin, Jichao/0000-0003-0311-9392 FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia National Laboratories is a multi program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 57 TC 5 Z9 5 U1 2 U2 37 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD NOV 1 PY 2013 VL 252 BP 86 EP 108 DI 10.1016/j.jcp.2013.06.012 PG 23 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA 194KZ UT WOS:000322633500006 ER PT J AU Arazi, A Pendergraft, WF Ribeiro, RM Perelson, AS Hacohen, N AF Arazi, Arnon Pendergraft, William F., III Ribeiro, Ruy M. Perelson, Alan S. Hacohen, Nir TI Human systems immunology: Hypothesis-based modeling and unbiased data-driven approaches SO SEMINARS IN IMMUNOLOGY LA English DT Review DE Systems immunology; Hypothesis-based modeling; Unbiased data-driven approaches; Dynamical modeling; Viral infections; Autoimmunity ID HEPATITIS-C VIRUS; T-CELL VACCINATION; DYNAMICS IN-VIVO; GENE-EXPRESSION PROFILES; IMMUNODEFICIENCY-VIRUS; HIV-1 INFECTION; MULTIPLE-SCLEROSIS; INSULIN SENSITIVITY; IMMUNE-SYSTEM; ANTIRETROVIRAL THERAPY AB Systems immunology is an emerging paradigm that aims at a more systematic and quantitative understanding of the immune system. Two major approaches have been utilized to date in this field: unbiased data-driven modeling to comprehensively identify molecular and cellular components of a system and their interactions; and hypothesis-based quantitative modeling to understand the operating principles of a system by extracting a minimal set of variables and rules underlying them. In this review, we describe applications of the two approaches to the study of viral infections and autoimmune diseases in humans, and discuss possible ways by which these two approaches can synergize when applied to human immunology. (C) 2012 Elsevier Ltd. All rights reserved. C1 [Pendergraft, William F., III; Hacohen, Nir] Massachusetts Gen Hosp, Ctr Immunol & Inflammatory Dis, Charlestown, MA 02129 USA. [Arazi, Arnon; Pendergraft, William F., III; Hacohen, Nir] Broad Inst MIT & Harvard, Cambridge Ctr 7, Cambridge, MA 02142 USA. [Pendergraft, William F., III; Hacohen, Nir] Harvard Univ, Sch Med, Dept Med, Boston, MA 02115 USA. [Pendergraft, William F., III] Massachusetts Gen Hosp, Dept Med, Div Nephrol, Boston, MA 02114 USA. [Ribeiro, Ruy M.; Perelson, Alan S.] Los Alamos Natl Lab, Theoret Biol & Biophys Grp, Los Alamos, NM 87545 USA. RP Perelson, AS (reprint author), Los Alamos Natl Lab, Theoret Biol & Biophys Grp, MS-K710, Los Alamos, NM 87545 USA. EM arnonar@broadinstitute.org; wpendergraft@partners.org; ruy@lanl.gov; asp@lanl.gov; nhacohen@partners.org OI Ribeiro, Ruy/0000-0002-3988-8241 FU U.S. Department of Energy [DE-AC52-06NA25396]; NIH [AI028433, OD011095, P20-RR018754, HHSN272201000055C]; New Innovator Award [OD002230, P50 HG006193, GM093080]; Foundation for Science and Technology of Portugal [PCOFUND-GA-2009-246542]; American Society of Nephrology FX Portions of this work were done under the auspices of the U.S. Department of Energy under contract DE-AC52-06NA25396 (AP) and supported by NIH grants AI028433 (AP), OD011095 (AP), P20-RR018754 (APRMR), New Innovator Award DP2 OD002230 (NH), P50 HG006193 (NH), GM093080 (NH), and NIH contract HHSN272201000055C (AP). RMR received partial funding from the Foundation for Science and Technology of Portugal (PCOFUND-GA-2009-246542). WFPIII is supported by a research fellowship from the American Society of Nephrology. NR 115 TC 9 Z9 9 U1 3 U2 9 PU ACADEMIC PRESS LTD- ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL RD, LONDON NW1 7DX, ENGLAND SN 1044-5323 J9 SEMIN IMMUNOL JI Semin. Immunol. PD OCT 31 PY 2013 VL 25 IS 3 BP 193 EP 200 DI 10.1016/j.smim.2012.11.003 PG 8 WC Immunology SC Immunology GA 257WS UT WOS:000327419100002 PM 23375135 ER PT J AU Polizos, G Vaia, RA Koerner, H Manias, E AF Polizos, Georgios Vaia, Richard A. Koerner, Hilmar Manias, Evangelos TI Dynamics of Amphiphilic Surfactants Confined in Montmorillonite Slits with Different Cation Exchange Capacities SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID LOW-FREQUENCY DISPERSION; POLYMER/LAYERED SILICATE NANOCOMPOSITES; POLYMER-CLAY NANOCOMPOSITES; MODIFIED LAYERED SILICATES; VITREOUS IONIC CONDUCTORS; DIELECTRIC-RELAXATION; MOLECULAR-DYNAMICS; ELECTRICAL-CONDUCTIVITY; COMPUTER-SIMULATION; COLLOIDAL PARTICLES AB Alkylammonium surfactants were nanoscopically confined between montmorillonite layers of varied negative surface charge, i.e., of varied cation exchange capacities. Dielectric relaxation spectroscopy was employed to probe the interfacial dynamics, arising from the mobility of the cations on the silicate surfaces, as a function of the confining walls' surface charge. Standard methods to dry the organo-silicates were employed; however, water was still detected physisorbed in the galleries; the dynamics of these water molecules were also detected and were found to be coupled with the dynamics of the ammoniums at high temperatures. A transition in the mobility of the cations, approximately at 75 degrees C (which is in good agreement with the conformational changes of the alkyl groups, reported in the literature), is observed, and a model is proposed on the basis of the dynamics of the confined water. Entropic contributions arising from variation in the surface charge density are also discussed in detail. The existence of water in the interlayer-in spite of drying the nanofillers in accordance to industrial practices and the interrelated surfactant/water dynamics bring forward important implications for the design and processing of polymer-based nanocomposites based on these fillers. C1 [Polizos, Georgios] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Vaia, Richard A.; Koerner, Hilmar; Manias, Evangelos] Mat & Mfg Directorate, Air Force Res Lab, Wright Patterson AFB, OH 45433 USA. [Polizos, Georgios; Manias, Evangelos] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. RP Polizos, G (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. EM polyzosg@ornl.gov; manias@psu.edu RI Manias, Evangelos/A-7557-2011 FU National Science Foundation [DMR-0602877]; US Air Force SFFP fellowship; U.S. Department of Energy, Office of Electricity Delivery and Energy Reliability - Power Electronics Program; U.S. Department of Energy [DE-AC05-00OR22725] FX This work was supported by the National Science Foundation (MWN grant, NSF Grant No. DMR-0602877); E.M.'s stay in AFRL was supported through an US Air Force SFFP fellowship, administered through NRC. Work was also supported by the U.S. Department of Energy, Office of Electricity Delivery and Energy Reliability - Power Electronics Program. Oak Ridge National Laboratory is operated for the U.S. Department of Energy by U.T.-Battelle under Contract No. DE-AC05-00OR22725. NR 99 TC 4 Z9 4 U1 0 U2 25 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 EI 1520-5207 J9 J PHYS CHEM B JI J. Phys. Chem. B PD OCT 31 PY 2013 VL 117 IS 43 BP 13667 EP 13678 DI 10.1021/jp4067845 PG 12 WC Chemistry, Physical SC Chemistry GA 247HM UT WOS:000326608500031 PM 24083909 ER PT J AU Chen, HA Hsin, CL Huang, YT Tang, ML Dhuey, S Cabrini, S Wu, WW Leone, SR AF Chen, Hsiang-An Hsin, Cheng-Lun Huang, Yu-Ting Tang, Ming Lee Dhuey, Scott Cabrini, Stefano Wu, Wen-Wei Leone, Stephen R. TI Measurement of Interlayer Screening Length of Layered Graphene by Plasmonic Nanostructure Resonances SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID SILVER NANOPARTICLES; RAMAN-SCATTERING; FILMS; SPECTROSCOPY; SUBSTRATE; DEVICES; SIO2 AB The variation in localized surface plasmon resonances of single Au nanodisks (diameter 100 nm and height 25 nm) on 0-13 graphene layers is investigated using dark-field scattering spectroscopy to obtain the graphene electric field screening length. For nanodisks (NDs) with and without underlying graphene layers on a SiO2 (300 nm)/Si substrate, the plasmon resonance red shifts from 604 to 620 nm with increasing graphene layers. The spectra of the plasmonic nanostructures obey an exponential saturation function versus increasing number of layers of graphene from 0 to 13. As a conducting film, the graphene layers screen the electric field generated by the plasmonic resonance of the Au NDs in the vicinity of the interface, and the red shifts of the resonance wavelength are explained in the framework of the electromagnetic field coupling between in-plane antiparallel image dipoles in the graphene layers and the ND dipole. A screening length of 1.2 +/- 0.2 nm, equivalent to 3-4 graphene layers, is experimentally obtained, in good agreement with the measurement by field-effect transistors and theoretical calculation in doped graphene. The resonance shift of plasmonic nanostructures on a layered graphene system provides an alternative and convenient method for screening length measurement of graphene films. C1 [Chen, Hsiang-An; Tang, Ming Lee; Leone, Stephen R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Hsin, Cheng-Lun] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Leone, Stephen R.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Hsin, Cheng-Lun] Natl Cent Univ, Dept Elect Engn, Tao Yuan 32001, Taiwan. [Huang, Yu-Ting; Wu, Wen-Wei] Natl Chiao Tung Univ, Dept Mat Sci & Engn, Hsinchu 30010, Taiwan. [Dhuey, Scott; Cabrini, Stefano] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Leone, Stephen R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Leone, SR (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM srl@berkeley.edu RI Foundry, Molecular/G-9968-2014 FU National Security Science and Engineering Faculty Fellowship; Air Force Office of Scientific Research [AFOSR-NSSEFF-FA9550-10-1-0195]; postdoctoral research abroad program; National Science Council, Taiwan [NSC100-2917-I-564-056, NCS 101-2218-E-008-014-MY2, NSC 100-2628-E-009-023-MY3]; Office of Science, Office of Basic Energy Sciences, Chemical Sciences Division of the U.S. Department of Energy [DE-AC02-05CH11231] FX The authors acknowledge Sarah Brittman for technical assistance and Terefe G. Habteyes for valuable discussions. This work is supported by a National Security Science and Engineering Faculty Fellowship, Air Force Office of Scientific Research under Grant No. AFOSR-NSSEFF-FA9550-10-1-0195, and postdoctoral research abroad program, National Science Council, Taiwan, under Contract No. NSC100-2917-I-564-056. Supplies and equipment are provided through the Materials Science Division (MSD) and Molecular Foundry, Lawrence Berkeley National Laboratory (LBNL), through support of the Director, Office of Science, Office of Basic Energy Sciences, Chemical Sciences Division of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Portions of the experimental supplies are provided by Cheng-Lun Hsin and Wen-Wei Wu under National Science Council, Taiwan, Grant No. NCS 101-2218-E-008-014-MY2 and No. NSC 100-2628-E-009-023-MY3, respectively. NR 38 TC 9 Z9 9 U1 2 U2 42 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 EI 1932-7455 J9 J PHYS CHEM C JI J. Phys. Chem. C PD OCT 31 PY 2013 VL 117 IS 43 BP 22211 EP 22217 DI 10.1021/jp312363x PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 247HJ UT WOS:000326608200007 ER PT J AU Lawton, TJ Pushkarev, V Wei, D Lucci, FR Sholl, DS Gellman, AJ Sykes, ECH AF Lawton, T. J. Pushkarev, V. Wei, D. Lucci, F. R. Sholl, D. S. Gellman, A. J. Sykes, E. C. H. TI Long Range Chiral Imprinting of Cu(110) by Tartaric Acid SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID ENANTIOSELECTIVE HETEROGENEOUS CATALYSIS; INITIO MOLECULAR-DYNAMICS; TOTAL-ENERGY CALCULATIONS; DIRECT STM EVIDENCE; WAVE BASIS-SET; METAL-SURFACES; ASYMMETRIC HYDROGENATION; (R,R)-TARTARIC ACID; ORGANIC-MOLECULES; FUNDAMENTAL INVESTIGATIONS AB Restructuring of metals by chiral molecules represents an important route to inducing and controlling enantioselective surface chemistry. Tartaric acid adsorption on Cu(110) has served as a useful system for understanding many aspects of chiral molecule adsorption and ordering on a metal surface, and a number of chiral and achiral unit cells have been reported. Herein, we show that given the appropriate annealing treatment, singly deprotonated tartaric acid monolayers can restructure the Cu metal itself, and that the resulting structure is both highly ordered and chiral. Molecular resolution scanning tunneling microscopy reveals that singly deprotonated tartaric acid extracts Cu atoms from the Cu(110) surface layer and incorporates them into highly ordered, chiral adatom arrays capped by a continuous molecular layer. Further evidence for surface restructuring comes from images of atom-deep trenches formed in the Cu(110) surface during the process. These trenches also run in low symmetry directions and are themselves chiral. Simulated scanning tunneling microscopy images are consistent with the appearance of the added atom rows and etched trenches. The chiral imprinting results in a long-range, highly ordered ((2)(6) (-1)(7)) unit cell covering the whole surface as confirmed by low energy electron diffraction. Details of the restructuring mechanism were further investigated via time-lapse imaging at elevated temperature. This work reveals the stages of nanoscale surface restructuring and offers an interesting method for chiral modification of an achiral metal surface. C1 [Lawton, T. J.; Lucci, F. R.; Sykes, E. C. H.] Tufts Univ, Dept Chem, Medford, MA 02155 USA. [Pushkarev, V.; Gellman, A. J.] Carnegie Mellon Univ, Dept Chem Engn, Pittsburgh, PA 15213 USA. [Wei, D.; Sholl, D. S.] Georgia Inst Technol, Sch Chem & Biomol Engn, Atlanta, GA 30332 USA. [Gellman, A. J.] US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. RP Sykes, ECH (reprint author), 62 Talbot Ave, Medford, MA 02155 USA. EM charles.sykes@tufts.edu RI Gellman, Andrew/M-2487-2014 OI Gellman, Andrew/0000-0001-6618-7427 FU National Science Foundation [CHE-1012358, CHE-1012307, CHE-1012524] FX This work has been supported by the National Science Foundation through a collaborative grant CHE-1012358 (V.P., A.J.G.), CHE-1012307 (T.J.L., E.C.H.S.) and CHE-1012524 (D.W., D.S.S.). NR 71 TC 20 Z9 20 U1 3 U2 77 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 EI 1932-7455 J9 J PHYS CHEM C JI J. Phys. Chem. C PD OCT 31 PY 2013 VL 117 IS 43 BP 22290 EP 22297 DI 10.1021/jp402015r PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 247HJ UT WOS:000326608200018 ER PT J AU Rosenberg, RA Symonds, JM Kalyanaraman, V Markus, T Orlando, TM Naaman, R Medina, EA Lopez, FA Mujica, V AF Rosenberg, Richard A. Symonds, Joshua M. Kalyanaraman, Vijayalakshmi Markus, Tal Orlando, Thomas M. Naaman, Ron Medina, Ernesto A. Lopez, Floralba A. Mujica, Vladimiro TI Kinetic Energy Dependence of Spin Filtering of Electrons Transmitted through Organized Layers of DNA SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID PHOTOELECTRON-SPECTROSCOPY; FILMS; TRANSMISSION; MONOLAYERS AB We present an experimental and theoretical study of the kinetic energy dependence of spin filtering of electrons by organized layers of DNA adsorbed on a gold substrate. When Au 4f(7/2,5/2) levels are ionized by circularly polarized X-rays, the emitted electrons will be spin polarized. The spin distribution depends on the particular sublevel and is opposite for right versus left circularly polarized light. If the DNA overlayer preferentially attenuates one spin over another, then there should be a circular dichroism (CD) in the X-ray photoelectron spectroscopy (XPS) spectra observed with the different polarizations. Using synchrotron radiation excitation, XPS CD measurements were made of electrons with kinetic energies in the range 30 to 760 eV. In all cases there was no evidence of any significant dichroism. These results are explained by a model in which the longitudinal polarization is strongly dependent on the k-vector, and hence the energy or the wavelength, which are simply connected to the magnitude of this vector of the incoming electrons. For a helix with a fixed number of turns, this dependence is due to a coherent process associated with multiple scattering. This model predicts that there is a window of energies where changes in the polarization should be expected. Two competing effects determine this window: The energy has to be small enough to allow for at least double scattering, but large enough so that the de Broglie wavelength probes the chiral structure. Also at very low energies the spin-orbit interaction weakens and no polarization results. C1 [Rosenberg, Richard A.; Kalyanaraman, Vijayalakshmi] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Symonds, Joshua M.; Orlando, Thomas M.] Georgia Inst Technol, Sch Chem & Biochem, Atlanta, GA 30332 USA. [Symonds, Joshua M.; Orlando, Thomas M.] Georgia Inst Technol, Sch Phys, Atlanta, GA 30332 USA. [Markus, Tal; Naaman, Ron] Weizmann Inst Sci, Dept Chem Phys, IL-76100 Rehovot, Israel. [Medina, Ernesto A.] Inst Venezolano Invest Cient, Ctr Fis, Lab Fis Estadist Sist Desordenados, Caracas 1020A, Venezuela. [Lopez, Floralba A.] Univ Los Andes, Dept Quim, Quimicofis Fluidos & Fenomenos Interfaci QUIFFIS, Merida 5101, Venezuela. [Mujica, Vladimiro] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Mujica, Vladimiro] Arizona State Univ, Dept Chem & Biochem, Tempe, AZ 85287 USA. [Mujica, Vladimiro] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. RP Rosenberg, RA (reprint author), Argonne Natl Lab, Adv Photon Source, 9700 S Cass Ave, Argonne, IL 60439 USA. EM rar@aps.anl.gov FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; National Science Foundation [DMR-0537588]; NSF [NSF CHE-1124895]; U.S. Department of Energy, Office of Science [DE-FG02-02ER15337]; Nir Eliyahu FX The work performed at the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Contract No. DE-AC02-06CH11357. This work is based in part upon research conducted at the Synchrotron Radiation Center, University of Wisconsin Madison, which is supported by the National Science Foundation under Award No. DMR-0537588. V.M. acknowledges the support of NSF through Award No. NSF CHE-1124895. T.M.O. and J.M.S. wish to acknowledge support from the U.S. Department of Energy, Office of Science, Contract No. DE-FG02-02ER15337. We would like to thank Nir Eliyahu for experimental support. NR 24 TC 6 Z9 6 U1 3 U2 30 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 EI 1932-7455 J9 J PHYS CHEM C JI J. Phys. Chem. C PD OCT 31 PY 2013 VL 117 IS 43 BP 22307 EP 22313 DI 10.1021/jp402387y PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 247HJ UT WOS:000326608200020 ER PT J AU Yaffe, O Ely, T Har-Lavan, R Egger, DA Johnston, S Cohen, H Kronik, L Vilan, A Cahen, D AF Yaffe, Omer Ely, Tal Har-Lavan, Rotem Egger, David A. Johnston, Steve Cohen, Hagai Kronik, Leeor Vilan, Ayelet Cahen, David TI Effect of Molecule-Surface Reaction Mechanism on the Electronic Characteristics and Photovoltaic Performance of Molecularly Modified Si SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID HYDROGEN-TERMINATED SILICON; SELF-ASSEMBLED MONOLAYERS; ORGANIC MONOLAYERS; ALKYL MONOLAYERS; AQUEOUS-SOLUTIONS; CURRENT TRANSPORT; SI(111) SURFACE; CHEMICAL-BOND; WORK FUNCTION; RECOMBINATION AB We report on the passivation properties of molecularly modified, oxide-free Si(111) surfaces. The reaction of 1-alcohol with the H-passivated Si(111) surface can follow two possible paths, nucleophilic substitution (S-N) and radical chain reaction (RCR), depending on adsorption conditions. Moderate heating leads to the SN reaction, whereas with UV irradiation RCR dominates, with SN as a secondary path. We show that the site-sensitive SN reaction leads to better electrical passivation, as indicated by smaller surface band bending and a longer lifetime of minority carriers. However, the surface-insensitive RCR reaction leads to more dense monolayers and, therefore, to much better chemical stability, with lasting protection of the Si surface against oxidation. Thus, our study reveals an inherent dissonance between electrical and chemical passivation. Alkoxy monolayers, formed under UV irradiation, benefit, though, from both chemical and electronic passivation because under these conditions both SN and RCR occur. This is reflected in longer minority carrier lifetimes, lower reverse currents in the dark, and improved photovoltaic performance, over what is obtained if only one of the mechanisms operates. These results show how chemical kinetics and reaction paths impact electronic properties at the device level. It further suggests an approach for effective passivation of other semiconductors. C1 [Yaffe, Omer; Ely, Tal; Har-Lavan, Rotem; Kronik, Leeor; Vilan, Ayelet; Cahen, David] Weizmann Inst Sci, Dept Mat & Interfaces, IL-76100 Rehovot, Israel. [Egger, David A.] Graz Univ Technol, Inst Solid State Phys, A-8010 Graz, Austria. [Johnston, Steve] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Cohen, Hagai] Weizmann Inst Sci, Dept Chem Res Support, IL-76100 Rehovot, Israel. RP Cahen, D (reprint author), Weizmann Inst Sci, Dept Mat & Interfaces, IL-76100 Rehovot, Israel. EM leeor.kronik@weizmann.ac.il; ayelet.vilan@weizmann.ac.il; david.cahen@weizmann.ac.il RI Egger, David/M-8926-2015 FU Israel Science Foundation; Wolfson family trust; Leona M. and Harry B. Helmsley Charitable Trust; Grand Centre for Sensors and Security; Kimmel Centre for Nanoscale Science; Austrian Academy of Sciences; Austrian Science Fund (FWF) [I937-N19]; Azrieli Foundation FX We thank Ofer Sinai, Ariel Biller, Pabitra Kumar Nayak (WIS), Chaim Sukenik (Bar-Ilan), J. Schwartz (Princeton), and Yves Chabal (UT Dallas) for useful discussions and guidance. A.V., L.K, and D.C. thank the Israel Science Foundation via its centres of Excellence program, for partial support. D.C. & L.K. thank the Wolfson family trust and the Leona M. and Harry B. Helmsley Charitable Trust, and D.C. thanks the Grand Centre for Sensors and Security and the Kimmel Centre for Nanoscale Science for support. L.K. thanks the Lise Meitner Minerva Center for Computational Chemistry. D.A.E. is a recipient of a DOC-fellowship by the Austrian Academy of Sciences, and further financial support by the Austrian Science Fund (FWF): I937-N19 is gratefully acknowledged. O.Y. thanks the Azrieli Foundation for the award of an Azrieli Fellowship. D.C. holds the Rowland and Sylvia Schaefer chair in Energy research. NR 78 TC 10 Z9 10 U1 0 U2 32 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD OCT 31 PY 2013 VL 117 IS 43 BP 22351 EP 22361 DI 10.1021/jp4027755 PG 11 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 247HJ UT WOS:000326608200025 ER PT J AU Lockyear, JF Welz, O Savee, JD Goulay, F Trevitt, AJ Taatjes, CA Osborn, DL Leone, SR AF Lockyear, Jessica F. Welz, Oliver Savee, John D. Goulay, Fabien Trevitt, Adam J. Taatjes, Craig A. Osborn, David L. Leone, Stephen R. TI Isomer Specific Product Detection in the Reaction of CH with Acrolein SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID SET MODEL CHEMISTRY; RING-DOWN SPECTROSCOPY; RATE CONSTANTS; LOW-PRESSURE; CAVITY RING; UNSATURATED-HYDROCARBONS; COMBUSTION CHEMISTRY; CARBONYL-COMPOUNDS; RADICAL REACTIONS; BRANCHING RATIOS AB The products formed in the reaction between the methylidene radical (CH) and acrolein (CH2=CHCHO) are probed at 4 Torr and 298 K employing tunable vacuum-ultraviolet synchrotron light and multiplexed photoionization mass-spectrometry. The data suggest a principal exit channel of H loss from the adduct to yield C4H4O, accounting for (78 +/- 10)% of the products. Examination of the photoionization spectra measured upon reaction of both CH and CD with acrolein reveals that the isomeric composition of the C4H4O product is (60 +/- 12)% 1,3-butadienal and (17 +/- 10)% furan. The remaining 23% of the possible C4H4O products cannot be accurately distinguished without more reliable photoionization spectra of the possible product isomers but most likely involves oxygenated butyne species. In addition, C2H2O and C3H4 are detected, which account for (14 +/- 10)% and (8 +10, -8)% of the products, respectively. The C2H2O photoionization spectrum matches that of ketene and the C3H4 signal is composed of (24 +/- 14)% allene and (76 +/- 22)% propyne, with an upper limit of 8% placed on the cyclopropene contribution. The reactive potential energy surface is also investigated computationally, coefficients are calculated with RRKM theory. These calculations predict overall branching fractions for 1,3-butadienal and furan of 27% and 12%, respectively, in agreement with the experimental results. In contrast, the calculations predict a prominent CO + 2-methylvinyl product channel that is at most a minor channel according to the experimental results. Studies with the CD radical strongly suggest that the title reaction proceeds predominantly via cycloaddition of the radical onto the C=O bond of acrolein, with cycloaddition to the C=C bond being the second most probable reactive mechanism. C1 [Lockyear, Jessica F.; Leone, Stephen R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Welz, Oliver; Savee, John D.; Taatjes, Craig A.; Osborn, David L.] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA. [Goulay, Fabien] W Virginia Univ, Dept Chem, Morgantown, WV 26506 USA. [Trevitt, Adam J.] Univ Wollongong, Sch Chem, Wollongong, NSW 2522, Australia. [Leone, Stephen R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Leone, Stephen R.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. RP Leone, SR (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM srl@berkeley.edu RI Trevitt, Adam/A-2915-2009; Welz, Oliver/C-1165-2013 OI Trevitt, Adam/0000-0003-2525-3162; Welz, Oliver/0000-0003-1978-2412 FU Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy at Lawrence Berkeley National Laboratory [DE-AC03-76SF0098]; West Virginia University; Australian Research Council [DP1094135]; International Synchrotron Access Program (ISAP); National Collaborative Research Infrastructure Strategy grant by the Federal Government of Australia; Division of Chemical Sciences, Geosciences, and Biosciences, the Office of Basic Energy Sciences, the U.S. Department of Energy; National Nuclear Security Administration [DE-AC04-94AL85000] FX The Advanced Light Source and Chemical Sciences Division (S.R.L. and J.F.L.) are supported by the Director, Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy under Contract No. DE-AC03-76SF0098 at Lawrence Berkeley National Laboratory. F.G. acknowledges West Virginia University for funding (start up package). A.J.T. acknowledges funding support from the Australian Research Council (DP1094135) and travel funding provided by the International Synchrotron Access Program (ISAP) managed by the Australian Synchrotron. The ISAP is funded by a National Collaborative Research Infrastructure Strategy grant provided by the Federal Government of Australia. We thank Mr. Howard Johnsen for technical support of this experiment. Sandia authors (O.W., J.D.S., D.L.O., and CAT.) and the instrumentation for this work are supported by the Division of Chemical Sciences, Geosciences, and Biosciences, the Office of Basic Energy Sciences, the U.S. Department of Energy. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the National Nuclear Security Administration under Contract Number DE-AC04-94AL85000. NR 84 TC 7 Z9 7 U1 3 U2 51 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 EI 1520-5215 J9 J PHYS CHEM A JI J. Phys. Chem. A PD OCT 31 PY 2013 VL 117 IS 43 BP 11013 EP 11026 DI 10.1021/jp407428v PG 14 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 247HL UT WOS:000326608400004 PM 24088057 ER PT J AU Lee, D Greenman, L Sarovar, M Whaley, KB AF Lee, Donghyun Greenman, Loren Sarovar, Mohan Whaley, K. Birgitta TI Ab Initio Calculation of Molecular Aggregation Effects: A Coumarin-343 Case Study SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID DENSITY-FUNCTIONAL THEORY; EXCITATION-ENERGY TRANSFER; COUPLED-CLUSTER METHODS; BASIS-SETS; ORBITAL METHODS; CONFIGURATION-INTERACTION; REACTION CENTERS; WAVE-FUNCTIONS; SYSTEMS; ACCURACY AB We present time-dependent density functional theory (TDDFT) calculations for single and dimerized Coumarin-343 molecules to investigate the quantum mechanical effects of chromophore aggregation in extended systems designed to function as a new generation of sensors and light-harvesting devices. Using the single-chromophore results, we describe the construction of effective Hamiltonians to predict the excitonic properties of aggregate systems. We compare the electronic coupling properties predicted by such effective Hamiltonians to those obtained from TDDFT calculations of dimers and to the coupling predicted by the transition density cube (TDC) method. We determine the accuracy of the dipole dipole approximation and TDC with respect to the separation distance and orientation of the dimers. In particular, we investigate the effects of including Coulomb coupling terms ignored in the typical tight-binding effective Hamiltonian. We also examine effects of orbital relaxation which cannot be captured by either of these models. C1 [Lee, Donghyun; Greenman, Loren; Whaley, K. Birgitta] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Sarovar, Mohan] Sandia Natl Labs, Livermore, CA 94550 USA. RP Whaley, KB (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM whaley@berkeley.edu FU NSF [CHE-0233882, CHE-0840505]; United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; DARPA QuBE (Quantum Effects in Biological Environments) program [N66001-10-1-4068] FX We thank Matthew Francis and Dan Finley for useful discussions on virus-templated assembly for light harvesting. We thank the Molecular Graphics and Computation Facility at UC-Berkeley for computational resources, which were made possible by the NSF under contract numbers CHE-0233882 and CHE-0840505. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the United States Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. Financial support for this research was provided by the DARPA QuBE (Quantum Effects in Biological Environments) program under contract number N66001-10-1-4068 and by the NSF (grants CHE-0233882 and CHE-0840505). NR 68 TC 6 Z9 6 U1 4 U2 21 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD OCT 31 PY 2013 VL 117 IS 43 BP 11072 EP 11085 DI 10.1021/jp405152h PG 14 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 247HL UT WOS:000326608400009 PM 24044623 ER PT J AU Ciappina, MF Lee, TG Pindzola, MS Colgan, J AF Ciappina, M. F. Lee, T. -G. Pindzola, M. S. Colgan, J. TI Nucleus-nucleus effects in differential cross sections for antiproton-impact ionization of H atoms SO PHYSICAL REVIEW A LA English DT Article ID HYDROGEN AB We investigate the differential cross sections for antiproton-impact ionization of H atoms within the framework of time-dependent close-coupling theory. A Fourier transform method is employed in order to extract the fully differential cross sections for a specific value of projectile momentum transfer. The method allows us to incorporate the information about the interaction between the incoming projectile and the target nucleus, the so-called nucleus-nucleus interaction, and to assess its effect on the fully differential cross sections and double differential cross sections in projectile variables. C1 [Ciappina, M. F.; Lee, T. -G.; Pindzola, M. S.] Auburn Univ, Dept Phys, Auburn, AL 36849 USA. [Colgan, J.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Ciappina, MF (reprint author), Auburn Univ, Dept Phys, Auburn, AL 36849 USA. RI Lee, Teck Ghee/D-5037-2012; OI Lee, Teck Ghee/0000-0001-9472-3194; Ciappina, Marcelo/0000-0002-1123-6460; Colgan, James/0000-0003-1045-3858 FU US Department of Energy (DOE); US National Science Foundation (NSF); DOE ERCAP award at the National Energy Research Scientific Computing Center in Oakland, California, USA FX This work was supported in part by grants from the US Department of Energy (DOE) and the US National Science Foundation (NSF). The computational work was carried out under a DOE ERCAP award at the National Energy Research Scientific Computing Center in Oakland, California, USA. We thank Igor Bray and Ilkhom Abdurakhmanov for sending us their CCC data. NR 20 TC 2 Z9 2 U1 0 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1050-2947 EI 1094-1622 J9 PHYS REV A JI Phys. Rev. A PD OCT 31 PY 2013 VL 88 IS 4 AR 042714 DI 10.1103/PhysRevA.88.042714 PG 6 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA 244LE UT WOS:000326389100007 ER PT J AU Guo, H He, Y Chien, CC Levin, K AF Guo, Hao He, Yan Chien, Chih-Chun Levin, K. TI Compressibility in strongly correlated superconductors and superfluids: From the BCS regime to Bose-Einstein condensates SO PHYSICAL REVIEW A LA English DT Article ID FERMI-GAS; UNIVERSAL THERMODYNAMICS; TEMPERATURE; CROSSOVER AB We present a theoretical study of the compressibility kappa in a Fermi gas with attractive contact interactions, providing predictions for the strongly attractive regime and the superfluid phase. Our work emphasizes the compressibility sum rule and gauge invariance as constraints on kappa, and we show how within a Gor'kov-based t-matrix approach, these can be satisfied in the normal phase when no approximations are made. For tractability, approximations must be introduced, and it is believed that thermodynamical approaches to kappa are more reliable than correlation-function-based schemes. Contrasting with other studies in the literature, we present thermodynamic calculations of kappa. As expected of an approximate approach, ours do not satisfy the compressibility sum rule. However, without adjusting parameters, they yield semiquantitative agreement with experiment and provide physical insight into similar results obtained via quantum Monte Carlo simulations. C1 [Guo, Hao] Southeast Univ, Dept Phys, Nanjing 211189, Jiangsu, Peoples R China. [He, Yan; Levin, K.] Univ Chicago, James Franck Inst, Chicago, IL 60637 USA. [He, Yan; Levin, K.] Univ Chicago, Dept Phys, Chicago, IL 60637 USA. [Chien, Chih-Chun] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Guo, H (reprint author), Southeast Univ, Dept Phys, Nanjing 211189, Jiangsu, Peoples R China. FU NSF-MRSEC [0820054]; National Natural Science Foundation (NSF) of China; NSF of Jiangsu Province [11204032, SBK201241926] FX We thank M. Zwierlein and A. Rancon for their help. K.L. and Y.H. are supported by NSF-MRSEC Grant No. 0820054. H.G. is supported by the National Natural Science Foundation (NSF) of China and the NSF of Jiangsu Province (Grants No. 11204032 and No. SBK201241926). C.C.C. thanks the U.S. DOE via the LANL/LDRD Program. NR 27 TC 4 Z9 4 U1 0 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1050-2947 EI 1094-1622 J9 PHYS REV A JI Phys. Rev. A PD OCT 31 PY 2013 VL 88 IS 4 AR 043644 DI 10.1103/PhysRevA.88.043644 PG 5 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA 244LE UT WOS:000326389100011 ER PT J AU Coh, S Tan, LZ Louie, SG Cohen, ML AF Coh, Sinisa Tan, Liang Z. Louie, Steven G. Cohen, Marvin L. TI Theory of the Raman spectrum of rotated double-layer graphene SO PHYSICAL REVIEW B LA English DT Article ID BILAYER GRAPHENE AB We study theoretically the Raman spectrum of the rotated double-layer graphene, consisting of two graphene layers rotated with respect to each other by an arbitrary angle.. We find a relatively simple dependence of the Raman G peak intensity on the angle.. On the other hand, the Raman 2D peak position, intensity, and width show a much more complicated dependence on the angle.. We account for all of these effects, including dependence on the incoming photon energy, in good agreement with the experimental data. We find that it is sufficient to include the interaction between the graphene layers on the electronic degrees of freedom (resulting in the occurrence of Van Hove singularities in the density of states). We assume that the phonon degrees of freedom are unaffected by the interaction between the layers. Furthermore, we decompose the Raman 2D peak into two components having very different linewidths; these widths are almost independent of the angle.. The change in the intensity and the peak position of one of these two components gives insight into the dependence of the overall Raman 2D peak features as a function of the angle.. Furthermore, we study the influence of the coherence on the Raman signal, and we separately study the influence of the interaction between the layers on the electron wave functions and energies. Additionally, we show regions in the phonon spectrum giving rise to the Raman 2D peak signal. This work provides an insight into the interplay between the mechanical degree of freedom (angle.) and the electronic degrees of freedom (singularities in the density of states) in rotated double-layer graphene. Additionally, this work provides a way to establish experimentally the value of the rotation angle. using Raman spectroscopy measurement. This procedure becomes even more robust if one repeats the Raman spectroscopy measurement with a different incoming photon energy. C1 [Coh, Sinisa] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Coh, S (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM sinisa@civet.berkeley.edu OI Tan, Liang Z/0000-0003-4724-6369 FU Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, US Department of Energy [DE-AC02-05CH11231]; National Science Foundation [DMR10-1006184]; Simons Foundation Fellowship in Theoretical Physics FX We thank G. Samsonidze for discussion and F. Mauri for sharing data on the calculated monolayer graphene phonon band structure. This work was supported by the Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, US Department of Energy under Contract No. DE-AC02-05CH11231 and by the National Science Foundation under Grant No. DMR10-1006184, which provided for continuum model calculations. S. G. L. acknowledges support of a Simons Foundation Fellowship in Theoretical Physics. Computational resources were provided by theNational Energy Research Scientific Computing Center, which is supported by the Office of Science of the U. S. Department of Energy. NR 33 TC 24 Z9 24 U1 10 U2 62 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 31 PY 2013 VL 88 IS 16 AR 165431 DI 10.1103/PhysRevB.88.165431 PG 15 WC Physics, Condensed Matter SC Physics GA 244LN UT WOS:000326390000006 ER PT J AU Garcia-Lekue, A Sanchez-Portal, D Arnau, A Wang, LW AF Garcia-Lekue, A. Sanchez-Portal, D. Arnau, A. Wang, L. W. TI Plane-wave based electron tunneling through field emission resonance states SO PHYSICAL REVIEW B LA English DT Article ID IMAGE-POTENTIAL STATES; METAL-SURFACES; INTERFEROMETRY; IDENTIFICATION; EXCITATIONS; INTERFACE; BARRIER; DECAY AB Field emission resonances (FERs) on Cu(100) surface are investigated by means of tunneling regime simulations performed with a plane-wave based transport calculation method. FERs are located near the surface and decay into the vacuum, and their accurate simulation requires a faithful description of vacuum states. This type of simulations is thus not possible using the popular transport methods based on atom-centered localized basis sets and the use of plane waves becomes important. We introduce a procedure to treat self-consistently (SC) the finite bias nonequilibrium problem in tunneling regime. Image potential effects are included in a semiempirical way within the SC calculation. Tunneling through FERs is studied following a practical strategy to approximate the inelastic transmission for states lying in the band gap of the surface. As our approach permits the use of any tip geometry, tip effects on the energy and wave functions of FERs are explored. The method reported here provides an ideal tool for the simulation of FERs aimed at the understanding of experimental STS (scanning tunneling spectroscopy) observations. C1 [Garcia-Lekue, A.; Sanchez-Portal, D.; Arnau, A.] Donostia Int Phys Ctr, E-20018 San Sebastian, Spain. [Garcia-Lekue, A.] Basque Fdn Sci, IKERBASQUE, E-48011 Bilbao, Spain. [Sanchez-Portal, D.; Arnau, A.] Ctr Mixto CSIC UPV, Ctr Fis Mat CFM MPC, San Sebastian, Spain. [Arnau, A.] Univ Basque Country, Fac Quim, Dpto Fis Mat, San Sebastian, Spain. [Wang, L. W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, Berkeley, CA 94720 USA. RP Garcia-Lekue, A (reprint author), Donostia Int Phys Ctr, Paseo Manuel Lardizabal 4, E-20018 San Sebastian, Spain. RI Sanchez-Portal, Daniel /E-5858-2010; DONOSTIA INTERNATIONAL PHYSICS CTR., DIPC/C-3171-2014; arnau, andres/H-7901-2012; CSIC-UPV/EHU, CFM/F-4867-2012 OI arnau, andres/0000-0001-5281-3212; FU Basque Departamento de Educacion and the UPV/EHU [IT-756-13]; Spanish Ministerio de Ciencia e Innovacioon [FIS2010-19609-C02-00]; ETORTEK program; Basque Departamento de Industria and the Diputacion Foral de Gipuzkoa; National Energy Research Scientific Computing Center (NERSC); US DOE/SC/BES [DE-AC02-05CH11231] FX We acknowledge support from the Basque Departamento de Educacion and the UPV/EHU (Grant No. IT-756-13), the Spanish Ministerio de Ciencia e Innovacioon (Grant No. FIS2010-19609-C02-00), and the ETORTEK program funded by the Basque Departamento de Industria and the Diputacion Foral de Gipuzkoa. It used the resources of the National Energy Research Scientific Computing Center (NERSC). L. W. Wang is supported by the US DOE/SC/BES under contract No. DE-AC02-05CH11231. NR 49 TC 1 Z9 1 U1 2 U2 20 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 31 PY 2013 VL 88 IS 15 AR 155441 DI 10.1103/PhysRevB.88.155441 PG 9 WC Physics, Condensed Matter SC Physics GA 244LL UT WOS:000326389800007 ER PT J AU Rincon, J Garcia, DJ Hallberg, K Vojta, M AF Rincon, Julian Garcia, Daniel J. Hallberg, K. Vojta, Matthias TI Quantum phase transition between one-channel and two-channel Kondo polarons SO PHYSICAL REVIEW B LA English DT Article ID DENSITY-MATRIX RENORMALIZATION; DIMENSIONAL ELECTRON-GAS; IMPURITY; STATE; METALS; MODEL AB For a mobile spin-1/2 impurity, coupled antiferromagnetically to a one-dimensional gas of fermions, perturbative ideas have been used to argue in favor of two-channel Kondo behavior of the impurity spin. Here we combine general considerations and extensive numerical simulations to show that the problem displays a novel quantum phase transition between two-channel and one-channel Kondo screening upon increasing the Kondo coupling. We construct a ground-state phase diagram and discuss the various nontrivial crossovers as well as possible experimental realizations. C1 [Rincon, Julian] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Garcia, Daniel J.; Hallberg, K.] Comis Nacl Energia Atom, Ctr Atom Bariloche, Inst Balseiro, RA-8400 San Carlos De Bariloche, Rio Negro, Argentina. [Garcia, Daniel J.; Hallberg, K.] Consejo Nacl Invest Cient & Tecn, RA-8400 San Carlos De Bariloche, Rio Negro, Argentina. [Vojta, Matthias] Tech Univ Dresden, Inst Theoret Phys, D-01062 Dresden, Germany. RP Rincon, J (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RI Vojta, Matthias/B-2298-2012; OI Garcia, Daniel Julio/0000-0001-6777-9184 FU DFG [FG 960]; German-Israeli Foundation; Early Career Research Program of US DOE; Heinrich-Hertz-Stiftung NRW FX We thank B. Alascio, P. Cornaglia, A. Feiguin, E. Fradkin, T. Giamarchi, and C. Vojta for discussions. This research was supported by the DFG (FG 960), the German-Israeli Foundation, and the Early Career Research Program of US DOE. M.V. also acknowledges support by the Heinrich-Hertz-Stiftung NRW and the hospitality of the Centro Atomico Bariloche, where part of this work was performed. NR 26 TC 1 Z9 1 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 31 PY 2013 VL 88 IS 14 AR 140407 DI 10.1103/PhysRevB.88.140407 PG 4 WC Physics, Condensed Matter SC Physics GA 244LH UT WOS:000326389400001 ER PT J AU Schumacher, D Steffen, A Voigt, J Schubert, J Bruckel, T Ambaye, H Lauter, V AF Schumacher, D. Steffen, A. Voigt, J. Schubert, J. Brueckel, Th. Ambaye, H. Lauter, V. TI Inducing exchange bias in La0.67Sr0.33MnO3-delta/SrTiO3 thin films by strain and oxygen deficiency SO PHYSICAL REVIEW B LA English DT Article ID MAGNETORESISTANCE; MANGANITES; STOICHIOMETRY; ANISOTROPY; OXIDES AB We present an exchange bias (EB) effect of variable size in La0.67Sr0.33MnO3-delta single and La0.67Sr0.33MnO3-delta/SrTiO3 (LSMO/STO) bilayers grown on STO substrates. Samples have been prepared by pulsed laser deposition (PLD) and high-pressure sputter deposition (HSD) in oxygen atmosphere at different oxygen pressures. Increased out-of-plane lattice parameters of the LSMO layers and reduced Curie temperatures indicate oxygen deficiencies in the samples grown at lower oxygen pressures. We found an increase of the EB and the coercive fields with decreasing oxygen pressure, whereas the growth at high pressures does not lead to an EB effect. The depth-sensitive method of polarized neutron reflectometry (PNR) reveals a region with drastically reduced, maybe even completely vanishing net magnetization in the LSMO layer at the interface to STO in the exchange-biased samples, but not in the non-exchanged-biased one. It is suggested that an antiferromagnetic structure is formed in this part of the LSMO thin film, which causes the EB effect in this system. An explanation based on the strain-doping phase diagram of LSMO is provided. Thus our findings open a route for tuning the EB effect by changing the oxygen vacancy concentrations. C1 [Schumacher, D.; Steffen, A.; Voigt, J.; Schubert, J.; Brueckel, Th.; Ambaye, H.; Lauter, V.] Julich Ctr Neutron Sci JCNS, D-52425 Julich, Germany. [Schumacher, D.; Steffen, A.; Voigt, J.; Schubert, J.; Brueckel, Th.; Ambaye, H.; Lauter, V.] JARA FIT, Peter Grunberg Inst PGI, D-52425 Julich, Germany. [Schumacher, D.; Steffen, A.; Voigt, J.; Schubert, J.; Brueckel, Th.; Ambaye, H.; Lauter, V.] Forschungszentrum Julich, D-52425 Julich, Germany. [Ambaye, H.; Lauter, V.] Oak Ridge Natl Lab, Neutron Sci Directorate, Spallat Neutron Source, Oak Ridge, TN 37831 USA. RP Schumacher, D (reprint author), Julich Ctr Neutron Sci JCNS, D-52425 Julich, Germany. RI Bruckel, Thomas/J-2968-2013; Schubert, Jurgen/K-9543-2013; Ambaye, Haile/D-1503-2016; OI Bruckel, Thomas/0000-0003-1378-0416; Schubert, Jurgen/0000-0003-0185-6794; Ambaye, Haile/0000-0002-8122-9952; Voigt, Jorg/0000-0002-6556-4961; Steffen, Alexandra/0000-0002-9802-438X NR 27 TC 15 Z9 15 U1 11 U2 103 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD OCT 31 PY 2013 VL 88 IS 14 AR 144427 DI 10.1103/PhysRevB.88.144427 PG 7 WC Physics, Condensed Matter SC Physics GA 244LH UT WOS:000326389400002 ER PT J AU Allmond, JM AF Allmond, J. M. TI Simple correlations between electric quadrupole moments of atomic nuclei SO PHYSICAL REVIEW C LA English DT Article ID MULTIPLE COULOMB-EXCITATION; EVEN-EVEN NUCLEI; PT-OS NUCLEI; OSMIUM ISOTOPES; HEXADECAPOLE VIBRATIONS; ROTATIONAL STATES; SHAPES; TRANSITION; PT-196; BEAM AB Measurements of nonyrast electric quadrupole moments (i.e., diagonal E2 matrix elements) of atomic nuclei are becoming widely available from multiple-step Coulomb excitation. It is shown that, where quadrupole-moment data exist, < 2(1)(+) parallel to E2 parallel to 2(1)(+) > + < 2(2)(+) parallel to E2 parallel to 2(2)(+) > approximate to 0 is observed across a wide range of masses, deformations, and first 2(+) energies. Nearly all of these quadrupole-moment data, particularly < 2(2)(+) parallel to E2 parallel to|2(2)(+), are from the past two decades with half of the data from the past decade. In addition, < 4(1)(+) parallel to E2 parallel to|4(1)(+)> + < 4(2)(+) parallel to E2 parallel to 4(2)(+) > parallel to + < 4(3)(+) parallel to E2 parallel to 4(3)(+)> approximate to 0 is observed within two standard deviations for three of the four existing measurements. Despite many and varying complexities in the structure details of the individual nuclei, the correlations in the quadrupole moments appear simple. C1 Oak Ridge Natl Lab, Joint Inst Heavy Ion Res, Oak Ridge, TN 37831 USA. RP Allmond, JM (reprint author), Oak Ridge Natl Lab, Joint Inst Heavy Ion Res, Oak Ridge, TN 37831 USA. OI Allmond, James Mitchell/0000-0001-6533-8721 FU Office of Nuclear Physics, U.S. Department of Energy; U.S. Department of Energy FX The author would like to thank D. G. Jenkins, T. Papenbrock, D. C. Radford, D. J. Rowe, A. E. Stuchbery, and J. L. Wood for fruitful discussions and useful comments on the manuscript. Research sponsored by the Office of Nuclear Physics, U.S. Department of Energy. The Joint Institute for Heavy Ion Research has as member institutions the University of Tennessee, Vanderbilt University, and the Oak Ridge National Laboratory; it is supported by the members and by the U.S. Department of Energy. NR 68 TC 4 Z9 4 U1 0 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD OCT 31 PY 2013 VL 88 IS 4 AR 041307 DI 10.1103/PhysRevC.88.041307 PG 6 WC Physics, Nuclear SC Physics GA 244LR UT WOS:000326390500001 ER PT J AU Nag, S Singh, AK Ragnarsson, I Hubel, H Al-Khatib, A Bringel, P Engelhardt, C Neusser-Neffgen, A Hagemann, GB Herskind, B Sletten, G Carpenter, MP Janssens, RVF Khoo, TL Lauritsen, T Clark, RM Fallon, P Benzoni, G Bracco, A Camera, F Chowdhury, P AF Nag, Somnath Singh, A. K. Ragnarsson, I. Huebel, H. Al-Khatib, A. Bringel, P. Engelhardt, C. Neusser-Neffgen, A. Hagemann, G. B. Herskind, B. Sletten, G. Carpenter, M. P. Janssens, R. V. F. Khoo, T. L. Lauritsen, T. Clark, R. M. Fallon, P. Benzoni, G. Bracco, A. Camera, F. Chowdhury, P. TI Collective and noncollective excitations in Te-122 SO PHYSICAL REVIEW C LA English DT Article ID HIGH-SPIN STATES; ROTATIONAL BANDS; SMOOTH TERMINATION; HOLE EXCITATIONS; OBLATE STATES; NUCLEI; COEXISTENCE; REGION AB High-spin states in Te-122 were populated in the reaction Se-82(Ca-48, alpha 4n) Te-122 at a beam energy of 200 MeV and gamma-ray coincidences weremeasured with the Gammasphere spectrometer. The previously known level scheme was extended to considerably higher spin. Maximally aligned states and several high-energy transitions feeding into some of these levels were observed. In addition, seven collective high-spin bands were discovered for the first time in this nucleus. The experimental results are compared with cranked Nilsson-Strutinsky model calculations and possible configuration assignments to the new high-spin structures are discussed. C1 [Nag, Somnath; Singh, A. K.] Indian Inst Technol, Dept Phys & Meteorol, IN-721302 Kharagpur, W Bengal, India. [Ragnarsson, I.] Lund Univ, Div Math Phys, LTH, S-221 Lund, Sweden. [Huebel, H.; Al-Khatib, A.; Bringel, P.; Engelhardt, C.; Neusser-Neffgen, A.] Univ Bonn, Helmholtz Inst Strahlen & Kernphys, D-53115 Bonn, Germany. [Hagemann, G. B.; Herskind, B.; Sletten, G.] Niels Bohr Inst, DK-2100 Copenhagen O, Denmark. [Carpenter, M. P.; Janssens, R. V. F.; Khoo, T. L.; Lauritsen, T.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Clark, R. M.; Fallon, P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Benzoni, G.; Bracco, A.; Camera, F.] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Bracco, A.; Camera, F.] Univ Milan, Dipartimento Fis, I-20133 Milan, Italy. [Chowdhury, P.] Univ Massachusetts Lowell, Dept Phys, Lowell, MA 01854 USA. RP Nag, S (reprint author), Indian Inst Technol, Dept Phys & Meteorol, IN-721302 Kharagpur, W Bengal, India. RI Carpenter, Michael/E-4287-2015; OI Carpenter, Michael/0000-0002-3237-5734; Camera, Franco/0000-0003-1731-4834; benzoni, giovanna/0000-0002-7938-0338 FU CSIR, India [09/081(0704)/2009-EMR-I]; DST, India [SR/S2/HEP-09/2005]; Swedish Science Research Council; German BMBF [06 BN 109]; Danish FNU Council for Natural Sciences; U.S. Department of Energy, Office of Nuclear Physics [DE-AC02-06CH11357, DE-AC03-76SF00098] FX The authors would like to thank the ATLAS and Gammasphere operations staff for their support. S. N. acknowledges financial support from CSIR, India, under Contract No. 09/081(0704)/2009-EMR-I and help from Dr. P. Singh. This work was supported by the DST, India, under Project No. SR/S2/HEP-09/2005, by the Swedish Science Research Council, by the German BMBF under Contract No. 06 BN 109, by the Danish FNU Council for Natural Sciences, and by the U.S. Department of Energy, Office of Nuclear Physics, under Contracts No. DE-AC02-06CH11357 and No. DE-AC03-76SF00098. NR 36 TC 4 Z9 4 U1 0 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD OCT 31 PY 2013 VL 88 IS 4 AR 044335 DI 10.1103/PhysRevC.88.044335 PG 13 WC Physics, Nuclear SC Physics GA 244LR UT WOS:000326390500005 ER PT J AU Wiringa, RB Pastore, S Pieper, SC Miller, GA AF Wiringa, R. B. Pastore, S. Pieper, Steven C. Miller, Gerald A. TI Charge-symmetry breaking forces and isospin mixing in Be-8 SO PHYSICAL REVIEW C LA English DT Article ID PROTON ELASTIC-SCATTERING; LIGHT-NUCLEI; PRECISION-MEASUREMENT; MONTE-CARLO; ASYMMETRY; VIOLATION AB We report Green's function Monte Carlo calculations of isospin-mixing (IM) matrix elements for the 2(+), 1(+), and 3(+) T = 0 and 1 pairs of states at 16-19 MeV excitation in Be-8. The realistic Argonne nu(18) (AV18) two-nucleon and Illinois-7 three-nucleon potentials are used to generate the nuclear wave functions. Contributions from the full electromagnetic interaction and strong class III charge-symmetry breaking (CSB) components of the AV18 potential are evaluated. We also examine two theoretically more complete CSB potentials based on rho-omega mixing, tuned to give the same neutron-neutron scattering length as AV18. The contribution of these different CSB potentials to the H-3-He-3, Li-7-Be-7, and Li-8-B-8 isovector energy differences is evaluated and reasonable agreement with experiment is obtained. Finally, for the Be-8 IM calculation we add the small class IV CSB terms coming from one-photon, one-pion, and one-rho exchange, as well as rho-omega mixing. The expectation values of the three CSB models vary by up to 20% in the isovector energy differences, but only by 10% or less in the IM matrix element. The total matrix element gives 85-90% of the experimental IM value of -145 keV for the 2(+) doublet, with about two thirds coming from the Coulomb interaction. We also report the IM matrix element to the first 2(+) state at 3 MeV excitation, which is the final state for various tests of the standard model for beta decay. C1 [Wiringa, R. B.; Pieper, Steven C.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Pastore, S.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Miller, Gerald A.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. RP Wiringa, RB (reprint author), Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. EM wiringa@anl.gov; pastores@mailbox.sc.edu; spieper@anl.gov; miller@phys.washington.edu RI Wiringa, Robert/M-4970-2015 FU US DOE, Office of Nuclear Physics [DE-AC02-06CH11357]; NUCLEI SciDAC program; US NSF [PHY-1068305]; US DOE [DE-FG02-97ER41014] FX We thank I. Brida for valuable input. The many-body calculations were performed on the parallel computers of the Laboratory Computing Resource Center, Argonne National Laboratory. The work of R.B.W. and S.C.P. is supported by the US DOE, Office of Nuclear Physics, under Contract No. DE-AC02-06CH11357, and by the NUCLEI SciDAC program, that of S. P. is supported by the US NSF under Grant No. PHY-1068305, and that of G. A. M. is supported by the US DOE under Contract No. DE-FG02-97ER41014. NR 37 TC 7 Z9 7 U1 0 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD OCT 31 PY 2013 VL 88 IS 4 AR 044333 DI 10.1103/PhysRevC.88.044333 PG 8 WC Physics, Nuclear SC Physics GA 244LR UT WOS:000326390500003 ER PT J AU Adamson, P Barr, G Bishai, M Blake, A Bock, GJ Bogert, D Cao, SV Cherdack, D Childress, S Coelho, JAB Corwin, L Cronin-Hennessy, D de Jong, JK Devan, AV Devenish, NE Diwan, MV Escobar, CO Evans, JJ Falk, E Feldman, GJ Frohne, MV Gallagher, HR Gomes, RA Goodman, MC Gouffon, P Graf, N Gran, R Grzelak, K Habig, A Hartnell, J Hatcher, R Himmel, A Holin, A Hylen, J Irwin, GM Isvan, Z James, C Jensen, D Kafka, T Kasahara, SMS Koizumi, G Kordosky, M Kreymer, A Lang, K Ling, J Litchfield, PJ Lucas, P Mann, WA Marshak, ML Mathis, M Mayer, N Medeiros, MM Mehdiyev, R Meier, JR Messier, MD Miller, WH Mishra, SR Sher, SM Moore, CD Mualem, L Mufson, S Musser, J Naples, D Nelson, JK Newman, HB Nichol, RJ Nowak, JA Oliver, WP Orchanian, M Pahlka, RB Paley, J Patterson, RB Pawloski, G Phan-Budd, S Plunkett, RK Qiu, X Radovic, A Rebel, B Rosenfeld, C Rubin, HA Sanchez, MC Schneps, J Schreckenberger, A Schreiner, P Sharma, R Sousa, A Tagg, N Talaga, RL Thomas, J Thomson, MA Toner, R Torretta, D Tzanakos, G Urheim, J Vahle, P Viren, B Weber, A Webb, RC White, C Whitehead, L Wojcicki, SG Zwaska, R AF Adamson, P. Barr, G. Bishai, M. Blake, A. Bock, G. J. Bogert, D. Cao, S. V. Cherdack, D. Childress, S. Coelho, J. A. B. Corwin, L. Cronin-Hennessy, D. de Jong, J. K. Devan, A. V. Devenish, N. E. Diwan, M. V. Escobar, C. O. Evans, J. J. Falk, E. Feldman, G. J. Frohne, M. V. Gallagher, H. R. Gomes, R. A. Goodman, M. C. Gouffon, P. Graf, N. Gran, R. Grzelak, K. Habig, A. Hartnell, J. Hatcher, R. Himmel, A. Holin, A. Hylen, J. Irwin, G. M. Isvan, Z. James, C. Jensen, D. Kafka, T. Kasahara, S. M. S. Koizumi, G. Kordosky, M. Kreymer, A. Lang, K. Ling, J. Litchfield, P. J. Lucas, P. Mann, W. A. Marshak, M. L. Mathis, M. Mayer, N. Medeiros, M. M. Mehdiyev, R. Meier, J. R. Messier, M. D. Miller, W. H. Mishra, S. R. Sher, S. Moed Moore, C. D. Mualem, L. Mufson, S. Musser, J. Naples, D. Nelson, J. K. Newman, H. B. Nichol, R. J. Nowak, J. A. Oliver, W. P. Orchanian, M. Pahlka, R. B. Paley, J. Patterson, R. B. Pawloski, G. Phan-Budd, S. Plunkett, R. K. Qiu, X. Radovic, A. Rebel, B. Rosenfeld, C. Rubin, H. A. Sanchez, M. C. Schneps, J. Schreckenberger, A. Schreiner, P. Sharma, R. Sousa, A. Tagg, N. Talaga, R. L. Thomas, J. Thomson, M. A. Toner, R. Torretta, D. Tzanakos, G. Urheim, J. Vahle, P. Viren, B. Weber, A. Webb, R. C. White, C. Whitehead, L. Wojcicki, S. G. Zwaska, R. CA MINOS Collaboration TI Search for flavor-changing non-standard neutrino interactions by MINOS SO PHYSICAL REVIEW D LA English DT Article ID LEPTON CHARGE; OSCILLATIONS AB We report new constraints on flavor-changing non-standard neutrino interactions from the MINOS experiment, in which neutrino versus antineutrino interactions can be distinguished on an event-by-event basis. We analyzed a combined set of beam neutrino and antineutrino data from the well-understood NuMI beam, and found no evidence for deviations from standard neutrino mixing. The observed energy spectra constrain the non-standard neutrino interactions parameter to the range -0.20 < epsilon(mu tau) < 0.07 (90%C.L.). C1 [Goodman, M. C.; Paley, J.; Phan-Budd, S.; Sanchez, M. C.; Schreiner, P.; Talaga, R. L.] Argonne Natl Lab, Argonne, IL 60439 USA. [Tzanakos, G.] Univ Athens, Dept Phys, GR-15771 Athens, Greece. [Bishai, M.; Diwan, M. V.; Isvan, Z.; Ling, J.; Viren, B.; Whitehead, L.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Himmel, A.; Mualem, L.; Newman, H. B.; Orchanian, M.; Patterson, R. B.] CALTECH, Lauritsen Lab, Pasadena, CA 91125 USA. [Blake, A.; Thomson, M. A.; Toner, R.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Coelho, J. A. B.; Escobar, C. O.] Univ Estadual Campinas, IFGW UNICAMP, BR-13083970 Campinas, SP, Brazil. [Sousa, A.] Univ Cincinnati, Dept Phys, Cincinnati, OH 45221 USA. [Adamson, P.; Bock, G. J.; Bogert, D.; Childress, S.; Hatcher, R.; Hylen, J.; James, C.; Jensen, D.; Koizumi, G.; Kreymer, A.; Lucas, P.; Sher, S. Moed; Moore, C. D.; Pahlka, R. B.; Plunkett, R. K.; Rebel, B.; Sharma, R.; Torretta, D.; Zwaska, R.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Gomes, R. A.; Medeiros, M. M.] Univ Fed Goias, Inst Fis, BR-74001970 Goiania, Go, Brazil. [Feldman, G. J.; Sousa, A.; Toner, R.] Harvard Univ, Dept Phys, Cambridge, MA 02138 USA. [Frohne, M. V.] Coll Holy Cross, Notre Dame, IN 46556 USA. [Whitehead, L.] Univ Houston, Dept Phys, Houston, TX 77204 USA. [Graf, N.; Rubin, H. A.; White, C.] IIT, Dept Phys, Chicago, IL 60616 USA. [Corwin, L.; Mayer, N.; Messier, M. D.; Mufson, S.; Musser, J.; Urheim, J.] Indiana Univ, Bloomington, IN 47405 USA. [Sanchez, M. C.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Evans, J. J.; Holin, A.; Nichol, R. J.; Radovic, A.; Thomas, J.] UCL, Dept Phys & Astron, London WC1E 6BT, England. [Evans, J. J.] Univ Manchester, Sch Phys & Astron, Manchester M13 9PL, Lancs, England. [Cronin-Hennessy, D.; Kasahara, S. M. S.; Litchfield, P. J.; Marshak, M. L.; Meier, J. R.; Miller, W. H.; Nowak, J. A.; Pawloski, G.; Schreckenberger, A.] Univ Minnesota, Minneapolis, MN 55455 USA. [Gran, R.; Habig, A.] Univ Minnesota, Dept Phys, Duluth, MN 55812 USA. [Tagg, N.] Otterbein Coll, Westerville, OH 43081 USA. [Barr, G.; de Jong, J. K.; Weber, A.] Univ Oxford, Subdept Particle Phys, Oxford OX1 3RH, England. [Isvan, Z.; Naples, D.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Litchfield, P. J.; Weber, A.] Sci & Technol Facil Council, Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Gouffon, P.] Univ Sao Paulo, Inst Fis, BR-05315970 Sao Paulo, Brazil. [Mishra, S. R.; Rosenfeld, C.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Irwin, G. M.; Pawloski, G.; Qiu, X.; Wojcicki, S. G.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Devenish, N. E.; Falk, E.; Hartnell, J.] Univ Sussex, Dept Phys & Astron, Brighton BN1 9QH, E Sussex, England. [Webb, R. C.] Texas A&M Univ, Dept Phys, College Stn, TX 77843 USA. [Cao, S. V.; Lang, K.; Mehdiyev, R.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Cherdack, D.; Coelho, J. A. B.; Gallagher, H. R.; Kafka, T.; Mann, W. A.; Mayer, N.; Oliver, W. P.; Schneps, J.] Tufts Univ, Dept Phys, Medford, MA 02155 USA. [Grzelak, K.] Univ Warsaw, Dept Phys, PL-00681 Warsaw, Poland. [Devan, A. V.; Kordosky, M.; Mathis, M.; Nelson, J. K.; Vahle, P.] Coll William & Mary, Dept Phys, Williamsburg, VA 23187 USA. RP Adamson, P (reprint author), Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. RI Gomes, Ricardo/B-6899-2008; Coelho, Joao/D-3546-2013; Evans, Justin/P-4981-2014; Gouffon, Philippe/I-4549-2012; Nowak, Jaroslaw/P-2502-2016; Ling, Jiajie/I-9173-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017 OI Weber, Alfons/0000-0002-8222-6681; Cao, Son/0000-0002-9046-5324; Hartnell, Jeffrey/0000-0002-1744-7955; Cherdack, Daniel/0000-0002-3829-728X; Gomes, Ricardo/0000-0003-0278-4876; Evans, Justin/0000-0003-4697-3337; Gouffon, Philippe/0000-0001-7511-4115; Nowak, Jaroslaw/0000-0001-8637-5433; Ling, Jiajie/0000-0003-2982-0670; FU U.S. DOE; United Kingdom STFC; U.S. NSF; State of Minnesota; University of Athens, Greece; Brazil's FAPESP; Brazil's CNPq; Brazil's CAPES; University of Minnesota FX This work was supported by the U.S. DOE; the United Kingdom STFC; the U.S. NSF; the State and University of Minnesota; the University of Athens, Greece; and Brazil's FAPESP, CNPq and CAPES. We are grateful to the Minnesota Department of Natural Resources, the crew of the Soudan Underground Lab, and the personnel of Fermilab for their contribution to this effort. NR 40 TC 20 Z9 20 U1 0 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD OCT 31 PY 2013 VL 88 IS 7 AR 072011 DI 10.1103/PhysRevD.88.072011 PG 6 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 244LY UT WOS:000326391400002 ER PT J AU Bae, T Jang, YC Jeong, H Jung, C Kim, HJ Kim, J Kim, J Kim, K Kim, S Lee, W Leem, J Sharpe, SR Yoon, B AF Bae, Taegil Jang, Yong-Chull Jeong, Hwancheol Jung, Chulwoo Kim, Hyung-Jin Kim, Jangho Kim, Jongjeong Kim, Kwangwoo Kim, Sunghee Lee, Weonjong Leem, Jaehoon Sharpe, Stephen R. Yoon, Boram CA SWME Collaboration TI Neutral kaon mixing from new physics: Matrix elements in N-f=2+1 lattice QCD SO PHYSICAL REVIEW D LA English DT Article ID OPERATORS; DELTA-S=2 AB We present results for matrix elements of Delta S = 2 four-fermion operators arising generically in models of new physics. These are needed to constrain such models using the measured values of epsilon(K) and Delta M-K. We use lattice QCD with 2 + 1 flavors of improved staggered fermions on lattices generated by the MILC Collaboration. We extrapolate to the continuum from three lattice spacings ranging down to a approximate to 0.045 fm. Total errors are similar to 5%-6%, arising primarily from our use of one-loop matching between lattice and continuum operators. For two of the matrix elements, our results disagree significantly from those obtained using different fermion discretizations. C1 [Bae, Taegil] Korea Inst Sci & Technol Informat, Taejon 305806, South Korea. [Jang, Yong-Chull; Jeong, Hwancheol; Kim, Jangho; Kim, Jongjeong; Kim, Kwangwoo; Kim, Sunghee; Lee, Weonjong; Leem, Jaehoon; Yoon, Boram] Seoul Natl Univ, FPRD, Lattice Gauge Theory Res Ctr, Seoul 151747, South Korea. [Jang, Yong-Chull; Jeong, Hwancheol; Kim, Jangho; Kim, Jongjeong; Kim, Kwangwoo; Kim, Sunghee; Lee, Weonjong; Leem, Jaehoon; Yoon, Boram] Seoul Natl Univ, CTP, Dept Phys & Astron, Seoul 151747, South Korea. [Jung, Chulwoo; Kim, Hyung-Jin] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Sharpe, Stephen R.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. RP Bae, T (reprint author), Korea Inst Sci & Technol Informat, Taejon 305806, South Korea. FU Creative Research Initiatives Progam of the NRF [2013-003454]; Korean government (MSIP); U.S. DOE [DE-AC02-98CH10886, DE-FG02-96ER40956]; KISTI supercomputing center [KSC-2012-G3-08]; Office of Science of the U.S. DOE FX We thank Claude Bernard for providing unpublished information. We thank Peter Boyle, Nicolas Garron, and Vittorio Lubicz for helpful discussion. W. L. is supported by the Creative Research Initiatives program (2013-003454) of the NRF grant funded by the Korean government (MSIP). C. J. and S. R. S. are supported in part by the U.S. DOE through Contract No. DE-AC02-98CH10886 and Grant No. DE-FG02-96ER40956, respectively. Computations for this work were carried out in part on the QCDOC computer of the USQCD Collaboration, funded by the Office of Science of the U.S. DOE. W. L. acknowledges support from the KISTI supercomputing center through the strategic support program (No. KSC-2012-G3-08). NR 25 TC 7 Z9 7 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD OCT 31 PY 2013 VL 88 IS 7 AR 071503 DI 10.1103/PhysRevD.88.071503 PG 5 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 244LY UT WOS:000326391400001 ER PT J AU Lees, JP Poireau, V Tisserand, V Grauges, E Palano, A Eigen, G Stugu, B Brown, DN Kerth, LT Kolomensky, YG Lee, M Lynch, G Koch, H Schroeder, T Hearty, C Mattison, TS McKenna, JA So, RY Khan, A Blinov, VE Buzykaev, AR Druzhinin, VP Golubev, VB Kravchenko, EA Onuchin, AP Serednyakov, SI Skovpen, YI Solodov, EP Todyshev, KY Yushkov, AN Kirkby, D Lankford, AJ Mandelkern, M Dey, B Gary, JW Long, O Vitug, GM Campagnari, C Sevilla, MF Hong, TM Kovalskyi, D Richman, JD West, CA Eisner, AM Lockman, WS Martinez, AJ Schumm, BA Seiden, A Chao, DS Cheng, CH Echenard, B Flood, KT Hitlin, DG Ongmongkolkul, P Porter, FC Andreassen, R Huard, Z Meadows, BT Sokoloff, MD Sun, L Bloom, PC Ford, WT Gaz, A Nauenberg, U Smith, JG Wagner, SR Ayad, R Toki, WH Spaan, B Schubert, KR Schwierz, R Bernard, D Verderi, M Playfer, S Bettoni, D Bozzi, C Calabrese, R Cibinetto, G Fioravanti, E Garzia, I Luppi, E Piemontese, L Santoro, V Baldini-Ferroli, R Calcaterra, A de Sangro, R Finocchiaro, G Martellotti, S Patteri, P Peruzzi, IM Piccolo, M Rama, M Zallo, A Contri, R Guido, E Lo Vetere, M Monge, MR Passaggio, S Patrignani, C Robutti, E Bhuyan, B Prasad, V Morii, M Adametz, A Uwer, U Lacker, HM Dauncey, PD Mallik, U Chen, C Cochran, J Meyer, WT Prell, S Rubin, AE Gritsan, AV Arnaud, N Davier, M Derkach, D Grosdidier, G Le Diberder, F Lutz, AM Malaescu, B Roudeau, P Stocchi, A Wormser, G Lange, DJ Wright, DM Coleman, JP Fry, JR Gabathuler, E Hutchcroft, DE Payne, DJ Touramanis, C Bevan, AJ Di Lodovico, F Sacco, R Cowan, G Bougher, J Brown, DN Davis, CL Denig, AG Fritsch, M Gradl, W Griessinger, K Hafner, A Prencipe, E Barlow, RJ Lafferty, GD Behn, E Cenci, R Hamilton, B Jawahery, A Roberts, DA Cowan, R Dujmic, D Sciolla, G Cheaib, R Patel, PM Robertson, SH Biassoni, P Neri, N Palombo, F Cremaldi, L Godang, R Sonnek, P Summers, DJ Nguyen, X Simard, M Taras, P De Nardo, G Monorchio, D Onorato, G Sciacca, C Martinelli, M Raven, G Jessop, CP LoSecco, JM Honscheid, K Kass, R Brau, J Frey, R Sinev, NB Strom, D Torrence, E Feltresi, E Margoni, M Morandin, M Posocco, M Rotondo, M Simi, G Simonetto, F Stroili, R Akar, S Ben-Haim, E Bomben, M Bonneaud, GR Briand, H Calderini, G Chauveau, J Leruste, P Marchiori, G Ocariz, J Sitt, S Biasini, M Manoni, E Pacetti, S Rossi, A Angelini, C Batignani, G Bettarini, S Carpinelli, M Casarosa, G Cervelli, A Forti, F Giorgi, MA Lusiani, A Oberhof, B Paoloni, E Perez, A Rizzo, G Walsh, JJ Pegna, DL Olsen, J Smith, AJS Faccini, R Ferrarotto, F Ferroni, F Gaspero, M Gioi, LL Piredda, G Bunger, C Grunberg, O Hartmann, T Leddig, T Voss, C Waldi, R Adye, T Olaiya, EO Wilson, FF Emery, S de Monchenault, GH Vasseur, G Yeche, C Anulli, F Aston, D Bard, DJ Benitez, JF Cartaro, C Convery, MR Dorfan, J Dubois-Felsmann, GP Dunwoodie, W Ebert, M Field, RC Fulsom, BG Gabareen, AM Graham, MT Hast, C Innes, WR Kim, P Kocian, ML Leith, DWGS Lewis, P Lindemann, D Lindquist, B Luitz, S Luth, V Lynch, HL MacFarlane, DB Muller, DR Neal, H Nelson, S Perl, M Pulliam, T Ratcliff, BN Roodman, A Salnikov, AA Schindler, RH Snyder, A Su, D Sullivan, MK Va'vra, J Wagner, AP Wang, WF Wisniewski, WJ Wittgen, M Wright, DH Wulsin, HW Ziegler, V Park, W Purohit, MV White, RM Wilson, JR Randle-Conde, A Sekula, SJ Bellis, M Burchat, PR Miyashita, TS Puccio, EMT Alam, MS Ernst, JA Gorodeisky, R Guttman, N Peimer, DR Soffer, A Spanier, SM Ritchie, JL Ruland, AM Schwitters, RF Wray, BC Izen, JM Lou, XC Bianchi, F De Mori, F Filippi, A Gamba, D Zambito, S Lanceri, L Vitale, L Martinez-Vidal, F Oyanguren, A Villanueva-Perez, P Ahmed, H Albert, J Banerjee, S Bernlochner, FU Choi, HHF King, GJ Kowalewski, R Lewczuk, MJ Lueck, T Nugent, IM Roney, JM Sobie, RJ Tasneem, N Gershon, TJ Harrison, PF Latham, TE Band, HR Dasu, S Pan, Y Prepost, R Wu, SL AF Lees, J. P. Poireau, V. Tisserand, V. Grauges, E. Palano, A. Eigen, G. Stugu, B. Brown, D. N. Kerth, L. T. Kolomensky, Yu. G. Lee, M. Lynch, G. Koch, H. Schroeder, T. Hearty, C. Mattison, T. S. McKenna, J. A. So, R. Y. Khan, A. Blinov, V. E. Buzykaev, A. R. Druzhinin, V. P. Golubev, V. B. Kravchenko, E. A. Onuchin, A. P. Serednyakov, S. I. Skovpen, Yu. I. Solodov, E. P. Todyshev, K. Yu. Yushkov, A. N. Kirkby, D. Lankford, A. J. Mandelkern, M. Dey, B. Gary, J. W. Long, O. Vitug, G. M. Campagnari, C. Sevilla, M. Franco Hong, T. M. Kovalskyi, D. Richman, J. D. West, C. A. Eisner, A. M. Lockman, W. S. Martinez, A. J. Schumm, B. A. Seiden, A. Chao, D. S. Cheng, C. H. Echenard, B. Flood, K. T. Hitlin, D. G. Ongmongkolkul, P. Porter, F. C. Andreassen, R. Huard, Z. Meadows, B. T. Sokoloff, M. D. Sun, L. Bloom, P. C. Ford, W. T. Gaz, A. Nauenberg, U. Smith, J. G. Wagner, S. R. Ayad, R. Toki, W. H. Spaan, B. Schubert, K. R. Schwierz, R. Bernard, D. Verderi, M. Playfer, S. Bettoni, D. Bozzi, C. Calabrese, R. Cibinetto, G. Fioravanti, E. Garzia, I. Luppi, E. Piemontese, L. Santoro, V. Baldini-Ferroli, R. Calcaterra, A. de Sangro, R. Finocchiaro, G. Martellotti, S. Patteri, P. Peruzzi, I. M. Piccolo, M. Rama, M. Zallo, A. Contri, R. Guido, E. Lo Vetere, M. Monge, M. R. Passaggio, S. Patrignani, C. Robutti, E. Bhuyan, B. Prasad, V. Morii, M. Adametz, A. Uwer, U. Lacker, H. M. Dauncey, P. D. Mallik, U. Chen, C. Cochran, J. Meyer, W. T. Prell, S. Rubin, A. E. Gritsan, A. V. Arnaud, N. Davier, M. Derkach, D. Grosdidier, G. Le Diberder, F. Lutz, A. M. Malaescu, B. Roudeau, P. Stocchi, A. Wormser, G. Lange, D. J. Wright, D. M. Coleman, J. P. Fry, J. R. Gabathuler, E. Hutchcroft, D. E. Payne, D. J. Touramanis, C. Bevan, A. J. Di Lodovico, F. Sacco, R. Cowan, G. Bougher, J. Brown, D. N. Davis, C. L. Denig, A. G. Fritsch, M. Gradl, W. Griessinger, K. Hafner, A. Prencipe, E. Barlow, R. J. Lafferty, G. D. Behn, E. Cenci, R. Hamilton, B. Jawahery, A. Roberts, D. A. Cowan, R. Dujmic, D. Sciolla, G. Cheaib, R. Patel, P. M. Robertson, S. H. Biassoni, P. Neri, N. Palombo, F. Cremaldi, L. Godang, R. Sonnek, P. Summers, D. J. Nguyen, X. Simard, M. Taras, P. De Nardo, G. Monorchio, D. Onorato, G. Sciacca, C. Martinelli, M. Raven, G. Jessop, C. P. LoSecco, J. M. Honscheid, K. Kass, R. Brau, J. Frey, R. Sinev, N. B. Strom, D. Torrence, E. Feltresi, E. Margoni, M. Morandin, M. Posocco, M. Rotondo, M. Simi, G. Simonetto, F. Stroili, R. Akar, S. Ben-Haim, E. Bomben, M. Bonneaud, G. R. Briand, H. Calderini, G. Chauveau, J. Leruste, Ph. Marchiori, G. Ocariz, J. Sitt, S. Biasini, M. Manoni, E. Pacetti, S. Rossi, A. Angelini, C. Batignani, G. Bettarini, S. Carpinelli, M. Casarosa, G. Cervelli, A. Forti, F. Giorgi, M. A. Lusiani, A. Oberhof, B. Paoloni, E. Perez, A. Rizzo, G. Walsh, J. J. Pegna, D. Lopes Olsen, J. Smith, A. J. S. Faccini, R. Ferrarotto, F. Ferroni, F. Gaspero, M. Gioi, L. Li Piredda, G. Buenger, C. Gruenberg, O. Hartmann, T. Leddig, T. Voss, C. Waldi, R. Adye, T. Olaiya, E. O. Wilson, F. F. Emery, S. de Monchenault, G. Hamel Vasseur, G. Yeche, Ch. Anulli, F. Aston, D. Bard, D. J. Benitez, J. F. Cartaro, C. Convery, M. R. Dorfan, J. Dubois-Felsmann, G. P. Dunwoodie, W. Ebert, M. Field, R. C. Fulsom, B. G. Gabareen, A. M. Graham, M. T. Hast, C. Innes, W. R. Kim, P. Kocian, M. L. Leith, D. W. G. S. Lewis, P. Lindemann, D. Lindquist, B. Luitz, S. Luth, V. Lynch, H. L. MacFarlane, D. B. Muller, D. R. Neal, H. Nelson, S. Perl, M. Pulliam, T. Ratcliff, B. N. Roodman, A. Salnikov, A. A. Schindler, R. H. Snyder, A. Su, D. Sullivan, M. K. Va'vra, J. Wagner, A. P. Wang, W. F. Wisniewski, W. J. Wittgen, M. Wright, D. H. Wulsin, H. W. Ziegler, V. Park, W. Purohit, M. V. White, R. M. Wilson, J. R. Randle-Conde, A. Sekula, S. J. Bellis, M. Burchat, P. R. Miyashita, T. S. Puccio, E. M. T. Alam, M. S. Ernst, J. A. Gorodeisky, R. Guttman, N. Peimer, D. R. Soffer, A. Spanier, S. M. Ritchie, J. L. Ruland, A. M. Schwitters, R. F. Wray, B. C. Izen, J. M. Lou, X. C. Bianchi, F. De Mori, F. Filippi, A. Gamba, D. Zambito, S. Lanceri, L. Vitale, L. Martinez-Vidal, F. Oyanguren, A. Villanueva-Perez, P. Ahmed, H. Albert, J. Banerjee, Sw. Bernlochner, F. U. Choi, H. H. F. King, G. J. Kowalewski, R. Lewczuk, M. J. Lueck, T. Nugent, I. M. Roney, J. M. Sobie, R. J. Tasneem, N. Gershon, T. J. Harrison, P. F. Latham, T. E. Band, H. R. Dasu, S. Pan, Y. Prepost, R. Wu, S. L. CA BaBar Collaboration TI Measurement of an excess of (B)over-bar -> D-(*) tau(-)(v)over-bar(tau) decays and implications for charged Higgs bosons SO PHYSICAL REVIEW D LA English DT Article ID HIGH-ENERGY-PHYSICS; B-MESON DECAYS; BABAR DETECTOR; FORM-FACTORS; MODEL AB Based on the full BABAR data sample, we report improved measurements of the ratios R(D) = B((B) over bar -> D tau(-)(v) over bar (tau))/B((B) over bar -> Dl(-)(v) over bar (l)) and R(D*) = B((B) over bar -> D*tau(-)(v) over bar (tau))/B((B) over bar -> D*l(-)(v) over bar (l)), where l refers to either an electron or muon. These ratios are sensitive to new physics contributions in the form of a charged Higgs boson. We measure R(D) = 0.440 +/- 0.058 +/- 0.042 and R(D*) = 0.332 +/- 0.024 +/- 0.018, which exceed the standard model expectations by 2.0 sigma and 2.7 sigma, respectively. Taken together, the results disagree with these expectations at the 3.4 sigma level. This excess cannot be explained by a charged Higgs boson in the type II two-Higgs-doublet model. Kinematic distributions presented here exclude large portions of the more general type III two-Higgs-doublet model, but there are solutions within this model compatible with the results. C1 [Lees, J. P.; Poireau, V.; Tisserand, V.] Univ Savoie, CNRS, IN2P3, Lab Annecy Le Vieux Phys Particules, F-74941 Annecy Le Vieux, France. [Grauges, E.] Univ Barcelona, Dept ECM, Fac Fis, E-08028 Barcelona, Spain. [Palano, A.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Palano, A.] Univ Bari, Dipartimento Fis, I-70126 Bari, Italy. 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[Angelini, C.; Batignani, G.; Bettarini, S.; Carpinelli, M.; Casarosa, G.; Cervelli, A.; Forti, F.; Giorgi, M. A.; Oberhof, B.; Paoloni, E.; Rizzo, G.] Univ Pisa, Dipartimento Fis, I-56127 Pisa, Italy. [Lusiani, A.] Scuola Normale Super Pisa, I-56127 Pisa, Italy. [Pegna, D. Lopes; Olsen, J.; Smith, A. J. S.] Princeton Univ, Princeton, NJ 08544 USA. [Faccini, R.; Ferrarotto, F.; Ferroni, F.; Gaspero, M.; Gioi, L. Li; Piredda, G.] Ist Nazl Fis Nucl, Sez Roma, I-00185 Rome, Italy. [Faccini, R.; Ferroni, F.; Gaspero, M.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Buenger, C.; Gruenberg, O.; Hartmann, T.; Leddig, T.; Voss, C.; Waldi, R.] Univ Rostock, D-18051 Rostock, Germany. [Adye, T.; Olaiya, E. O.; Wilson, F. F.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Emery, S.; de Monchenault, G. Hamel; Vasseur, G.; Yeche, Ch.] CEA, Irfu, SPP, Ctr Saclay, F-91191 Gif Sur Yvette, France. [Anulli, F.; Aston, D.; Bard, D. J.; Benitez, J. F.; Cartaro, C.; Convery, M. R.; Dorfan, J.; Dubois-Felsmann, G. P.; Dunwoodie, W.; Ebert, M.; Field, R. C.; Fulsom, B. G.; Gabareen, A. M.; Graham, M. T.; Hast, C.; Innes, W. R.; Kim, P.; Kocian, M. L.; Leith, D. W. G. S.; Lewis, P.; Lindemann, D.; Lindquist, B.; Luitz, S.; Luth, V.; Lynch, H. L.; MacFarlane, D. B.; Muller, D. R.; Neal, H.; Nelson, S.; Perl, M.; Pulliam, T.; Ratcliff, B. N.; Roodman, A.; Salnikov, A. A.; Schindler, R. H.; Snyder, A.; Su, D.; Sullivan, M. K.; Va'vra, J.; Wagner, A. P.; Wang, W. F.; Wisniewski, W. J.; Wittgen, M.; Wright, D. H.; Wulsin, H. W.; Ziegler, V.] SLAC Natl Accelerator Lab, Stanford, CA 94309 USA. [Park, W.; Purohit, M. V.; White, R. M.; Wilson, J. R.] Univ S Carolina, Columbia, SC 29208 USA. [Randle-Conde, A.; Sekula, S. J.] So Methodist Univ, Dallas, TX 75275 USA. [Bellis, M.; Burchat, P. R.; Miyashita, T. S.; Puccio, E. M. T.] Stanford Univ, Stanford, CA 94305 USA. [Alam, M. S.; Ernst, J. A.] SUNY Albany, New York, NY 12222 USA. [Gorodeisky, R.; Guttman, N.; Peimer, D. R.; Soffer, A.] Tel Aviv Univ, Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Spanier, S. M.] Univ Tennessee, Knoxville, TN 37996 USA. [Ritchie, J. L.; Ruland, A. M.; Schwitters, R. F.; Wray, B. C.] Univ Texas Austin, Austin, TX 78712 USA. [Izen, J. M.; Lou, X. C.] Univ Texas Dallas, Richardson, TX 75083 USA. [Bianchi, F.; De Mori, F.; Filippi, A.; Gamba, D.; Zambito, S.] Ist Nazl Fis Nucl, Sez Torino, Turin, Italy. [Bianchi, F.; De Mori, F.; Gamba, D.; Zambito, S.] Univ Turin, Dipartimento Fis Sperimentale, I-10125 Turin, Italy. [Lanceri, L.; Vitale, L.] Ist Nazl Fis Nucl, Sez Trieste, I-34127 Trieste, Italy. [Lanceri, L.; Vitale, L.] Univ Trieste, Dipartimento Fis, I-34127 Trieste, Italy. [Martinez-Vidal, F.; Oyanguren, A.; Villanueva-Perez, P.] Univ Valencia, CSIC, IFIC, E-46071 Valencia, Spain. [Ahmed, H.; Albert, J.; Banerjee, Sw.; Bernlochner, F. U.; Choi, H. H. F.; King, G. J.; Kowalewski, R.; Lewczuk, M. J.; Lueck, T.; Nugent, I. M.; Roney, J. M.; Sobie, R. J.; Tasneem, N.] Univ Victoria, Victoria, BC V8W 3P6, Canada. [Gershon, T. J.; Harrison, P. F.; Latham, T. E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Band, H. R.; Dasu, S.; Pan, Y.; Prepost, R.; Wu, S. L.] Univ Wisconsin, Madison, WI 53706 USA. [Godang, R.] Univ S Alabama, Mobile, AL 36688 USA. RP Lees, JP (reprint author), Univ Savoie, CNRS, IN2P3, Lab Annecy Le Vieux Phys Particules, F-74941 Annecy Le Vieux, France. RI Morandin, Mauro/A-3308-2016; Lusiani, Alberto/A-3329-2016; Di Lodovico, Francesca/L-9109-2016; Calcaterra, Alessandro/P-5260-2015; Frey, Raymond/E-2830-2016; Lo Vetere, Maurizio/J-5049-2012; Lusiani, Alberto/N-2976-2015; Patrignani, Claudia/C-5223-2009; Monge, Maria Roberta/G-9127-2012; Forti, Francesco/H-3035-2011; Oyanguren, Arantza/K-6454-2014; Luppi, Eleonora/A-4902-2015; White, Ryan/E-2979-2015; Kravchenko, Evgeniy/F-5457-2015; Calabrese, Roberto/G-4405-2015; Martinez Vidal, F*/L-7563-2014; Kolomensky, Yury/I-3510-2015 OI Morandin, Mauro/0000-0003-4708-4240; Lusiani, Alberto/0000-0002-6876-3288; Di Lodovico, Francesca/0000-0003-3952-2175; Calcaterra, Alessandro/0000-0003-2670-4826; Frey, Raymond/0000-0003-0341-2636; Lo Vetere, Maurizio/0000-0002-6520-4480; Lusiani, Alberto/0000-0002-6876-3288; Patrignani, Claudia/0000-0002-5882-1747; Monge, Maria Roberta/0000-0003-1633-3195; Forti, Francesco/0000-0001-6535-7965; Oyanguren, Arantza/0000-0002-8240-7300; Luppi, Eleonora/0000-0002-1072-5633; White, Ryan/0000-0003-3589-5900; Calabrese, Roberto/0000-0002-1354-5400; Martinez Vidal, F*/0000-0001-6841-6035; Kolomensky, Yury/0000-0001-8496-9975 FU Natural Sciences and Engineering Research Council (Canada); Commissariat a l'Energie Atomique and Institut National de Physique Nucleaire et de Physique des Particules (France); Bundesministerium fur Bildung und Forschung and Deutsche Forschungsgemeinschaft (Germany); Istituto Nazionale di Fisica Nucleare (Italy); Foundation for Fundamental Research on Matter (Netherlands); Research Council of Norway; Ministry of Education and Science of the Russian Federation; Science and Technology Facilities Council (United Kingdom); Marie-Curie IEF program (European Union); A. P. Sloan Foundation (USA); U.S. Department of Energy and National Science Foundation; Ministerio de Economia y Competitividad (Spain) FX The concept for this analysis is to a large degree based on earlier BABAR work and we acknowledge the guidance provided by M. Mazur. The authors consulted with theorists A. Datta, S. Westhoff, S. Fajfer, J. Kamenik, and I. Nisandzic on the calculations of the charged Higgs contributions to the decay rates. We are grateful for the extraordinary contributions of our PEP-II colleagues in achieving the excellent luminosity and machine conditions that have made this work possible. The success of this project also relied critically on the expertise and dedication of the computing organizations that support BABAR. The collaborating institutions wish to thank SLAC for its support and the kind hospitality extended to them. This work is supported by the U.S. Department of Energy and National Science Foundation, the Natural Sciences and Engineering Research Council (Canada), the Commissariat a l'Energie Atomique and Institut National de Physique Nucleaire et de Physique des Particules (France), the Bundesministerium fur Bildung und Forschung and Deutsche Forschungsgemeinschaft (Germany), the Istituto Nazionale di Fisica Nucleare (Italy), the Foundation for Fundamental Research on Matter (Netherlands), the Research Council of Norway, the Ministry of Education and Science of the Russian Federation, Ministerio de Economia y Competitividad (Spain), and the Science and Technology Facilities Council (United Kingdom). Individuals have received support from the Marie-Curie IEF program (European Union) and the A. P. Sloan Foundation (USA). NR 47 TC 90 Z9 90 U1 1 U2 21 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD OCT 31 PY 2013 VL 88 IS 7 AR 072012 DI 10.1103/PhysRevD.88.072012 PG 30 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 244LY UT WOS:000326391400003 ER PT J AU Griest, K Cieplak, AM Lehner, MJ AF Griest, Kim Cieplak, Agnieszka M. Lehner, Matthew J. TI New Limits on Primordial Black Hole Dark Matter from an Analysis of Kepler Source Microlensing Data SO PHYSICAL REVIEW LETTERS LA English DT Article ID GALACTIC HALO; MAGELLANIC CLOUDS; MACHO PROJECT; STARS AB We present new limits on the allowed masses of a dark matter (DM) halo consisting of primordial black holes (PBH) (or any other massive compact halo object). We analyze two years of data from the Kepler satellite, searching for short-duration bumps caused by gravitational microlensing. After removing background events consisting of variable stars, flare events, and comets or asteroids moving through the Kepler field, we find no microlensing candidates. We measure the efficiency of our selection criteria by adding millions of simulated microlensing lensing events into the Kepler light curves. We find that PBH DM with masses in the range 2 x 10(-9)M(circle dot) to 10(-7)M(circle dot) cannot make up the entirety of the DM in the Milky Way. At the low-mass end, this decreases the allowed mass range by more than an order of magnititude. C1 [Griest, Kim; Cieplak, Agnieszka M.] Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. [Lehner, Matthew J.] Acad Sinica, Inst Astron & Astrophys, Taipei 106, Taiwan. [Lehner, Matthew J.] Univ Penn, Dept Phys & Astron, Philadelphia, PA 19104 USA. [Cieplak, Agnieszka M.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. RP Griest, K (reprint author), Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. EM kgriest@ucsd.edu; acieplak@ucsd.edu; mlehner@asiaa.sinica.edu.tw OI Lehner, Matthew/0000-0003-4077-0985 FU DOE [DE-FG03-97ER40546, DE-SC0009919]; National Science Foundation Graduate Research Fellowship [DGE0707423]; NASA [NAS5-26555]; NASA Office of Space Science [NNX09AF08G] FX K. G. and A. M. C. were supported in part by the DOE under Grants No. DE-FG03-97ER40546 and No. DE-SC0009919. A. M. C. was supported in part by the National Science Foundation Graduate Research Fellowship under Grant No. DGE0707423. Some of the data presented in this Letter were obtained from the Multimission Archive at the Space Telescope Science Institute (MAST). STScI is operated by the Association of Universities for Research in Astronomy, Inc., under NASA Contract No. NAS5-26555. Support for MAST for non-HST data is provided by the NASA Office of Space Science via Grant No. NNX09AF08G and by other grants and contracts. NR 29 TC 26 Z9 26 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 31 PY 2013 VL 111 IS 18 AR 181302 DI 10.1103/PhysRevLett.111.181302 PG 5 WC Physics, Multidisciplinary SC Physics GA 244ML UT WOS:000326393000004 PM 24237504 ER PT J AU Plechaty, C Presura, R Esaulov, AA AF Plechaty, C. Presura, R. Esaulov, A. A. TI Focusing of an Explosive Plasma Expansion in a Transverse Magnetic Field SO PHYSICAL REVIEW LETTERS LA English DT Article ID LASER-PRODUCED PLASMA; HYBRID-DRIFT INSTABILITY; JETS; MECHANISM; MOTION; SPACE AB The dynamics of a laser ablation plasma expanding in an external magnetic field have been investigated with imaging interferometry and shadowgraphy. The diagnostics reveal a new interaction mechanism, namely, the redirection of the explosive plasma expansion into a converging flow. A comparison with three-dimensional ideal magnetohydrodynamic simulation results supports the observation that the efficient lateral plasma confinement causes the plasma to converge on the axis and initiate a directed flow. The resulting collimated flow propagates across the magnetic field in a kinetic regime, which cannot be modeled within the same framework. C1 [Plechaty, C.; Presura, R.; Esaulov, A. A.] Univ Nevada, Reno, NV 89557 USA. RP Plechaty, C (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. EM plechaty5@llnl.gov; presura@unr.edu; esaulov@unr.edu FU U.S. DOE [DE-FC52-06NA27616] FX The authors would like to thank Dr. Sandra Stein, Leela O'Brien, Showera Haque, and Matthew Tooth for their help during the experiment, and Dr. Gennady Sarkisov for designing the interferometry and shadow diagnostics. This work was performed at the Nevada Terawatt Facility and supported by the U.S. DOE under Cooperative Agreement No. DE-FC52-06NA27616. NR 25 TC 11 Z9 11 U1 4 U2 16 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 31 PY 2013 VL 111 IS 18 AR 185002 DI 10.1103/PhysRevLett.111.185002 PG 5 WC Physics, Multidisciplinary SC Physics GA 244ML UT WOS:000326393000009 PM 24237528 ER PT J AU Hu, Q Xu, DH Zhou, Y Peng, RW Fan, RH Fang, NX Wang, QJ Huang, XR Wang, M AF Hu, Qing Xu, Di-Hu Zhou, Yu Peng, Ru-Wen Fan, Ren-Hao Fang, Nicholas X. Wang, Qian-Jin Huang, Xian-Rong Wang, Mu TI Position-sensitive spectral splitting with a plasmonic nanowire on silicon chip SO SCIENTIFIC REPORTS LA English DT Article ID GRATING COUPLERS; ON-INSULATOR; SILVER NANOWIRES; WAVE-GUIDES; LIGHT; PROPAGATION; TECHNOLOGY; DETECTOR; MICROSCOPY; PHOTONICS AB On-chip nanophotonics serves as the foundation for the new generation of information technology, but it is challenged by the diffraction limit of light. With the capabilities of confining light into (deep) subwavelength volumes, plasmonics makes it possible to dramatically miniaturize optical devices so as to integrate them into silicon chips. Here we demonstrate that by cascading nano-corrugation gratings with different periodicities on silver nanowires atop silicon, different colors can be spatially separated and chronologically released at different grating junctions. The released light frequency depends on the grating arrangement and corrugation periodicities. Hence the nanowire acts as a spectral splitter for sorting/demultiplexing photons at different nano-scale positions with a ten-femtosecond-level interval. Such nanowires can be constructed further into compact 2D networks or circuits. We believe that this study provides a new and promising approach for realizing spatiotemporal-sensitive spectral splitting and optical signal processing on nanoscales, and for general integration of nanophotonics with microelectronics. C1 [Hu, Qing; Xu, Di-Hu; Zhou, Yu; Peng, Ru-Wen; Fan, Ren-Hao; Wang, Qian-Jin; Wang, Mu] Nanjing Univ, Natl Lab Solid State Microstruct, Nanjing 210093, Jiangsu, Peoples R China. [Hu, Qing; Xu, Di-Hu; Zhou, Yu; Peng, Ru-Wen; Fan, Ren-Hao; Wang, Qian-Jin; Wang, Mu] Nanjing Univ, Dept Phys, Nanjing 210093, Jiangsu, Peoples R China. [Hu, Qing; Fang, Nicholas X.] MIT, Dept Mech Engn, Cambridge, MA 02139 USA. [Huang, Xian-Rong] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Wang, M (reprint author), Nanjing Univ, Natl Lab Solid State Microstruct, Nanjing 210093, Jiangsu, Peoples R China. EM rwpeng@nju.edu.cn; muwang@nju.edu.cn RI Fang, Nicholas/A-5856-2008; Arumugam, Thirumagal/C-3408-2014 OI Fang, Nicholas/0000-0001-5713-629X; FU Ministry of Science and Technology of China [2012CB921502, 2010CB630705]; National Science Foundation of China [11034005, 61077023, 11021403]; Ministry of Education of China [20100091110029]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; NSF [CMMI-1120724] FX This work was supported by the Ministry of Science and Technology of China (Grant Nos. 2012CB921502 and 2010CB630705), the National Science Foundation of China (Grant Nos. 11034005, 61077023, and 11021403), and partly by the Ministry of Education of China (20100091110029). XRH was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NXF acknowledges partial support by NSF Grant no. CMMI-1120724. NR 57 TC 16 Z9 17 U1 4 U2 52 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD OCT 31 PY 2013 VL 3 AR 3095 DI 10.1038/srep03095 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 243QZ UT WOS:000326333300004 PM 24172838 ER PT J AU Ma, CR Liu, M Chen, CL Lin, Y Li, YR Horwitz, JS Jiang, JC Meletis, EI Zhang, QY AF Ma, Chunrui Liu, Ming Chen, Chonglin Lin, Yuan Li, Yanrong Horwitz, J. S. Jiang, Jiechao Meletis, E. I. Zhang, Qingyu TI The Origin of Local Strain in Highly Epitaxial Oxide Thin Films SO SCIENTIFIC REPORTS LA English DT Article ID DIELECTRIC-PROPERTIES; TRANSPORT-PROPERTIES; 001 MGO; MAGNETORESISTANCE; FERROELECTRICITY; SRTIO3; HETEROSTRUCTURES; SURFACES AB The ability to control the microstructures and physical properties of hetero-epitaxial functional oxide thin films and artificial structures is a long-sought goal in functional materials research. Normally, only the lattice misfit between the film and the substrate is considered to govern the physical properties of the epitaxial films. In fact, the mismatch of film unit cell arrangement and the Surface-Step-Terrace (SST) dimension of the substrate, named as "SST residual matching", is another key factor that significantly influence the properties of the epitaxial film. The nature of strong local strain induced from both lattice mismatch and the SST residual matching on ferroelectric (Ba,Sr)TiO3 and ferromagnetic (La,Ca) MnO3 thin films are systematically investigated and it is demonstrated that this combined effect has a dramatic impact on the physical properties of highly epitaxial oxide thin films. A giant anomalous magnetoresistance effect (similar to 10(10)) was achieved from the as-designed vicinal surfaces. C1 [Ma, Chunrui; Chen, Chonglin] Univ Texas San Antonio, Dept Phys & Astron, San Antonio, TX 78249 USA. [Liu, Ming] Xi An Jiao Tong Univ, Minist Educ, Key Lab, Elect Mat Res Lab, Xian 710049, Peoples R China. [Liu, Ming] Xi An Jiao Tong Univ, Int Ctr Dielect Res, Xian 710049, Peoples R China. [Chen, Chonglin] Univ Houston, Texas Ctr Superconduct, Houston, TX 77204 USA. [Lin, Yuan; Li, Yanrong] Univ Elect Sci & Technol China, State Key Lab Elect Thin Films & Integrated Devic, Chengdu 610054, Sichuan, Peoples R China. [Horwitz, J. S.] US DOE, Germantown, MD 20585 USA. [Jiang, Jiechao; Meletis, E. I.] Univ Texas Arlington, Arlington, TX 76019 USA. [Zhang, Qingyu] Dalian Univ Technol, Key Lab Mat Modificat Laser, Dalian 116024, Peoples R China. RP Chen, CL (reprint author), Univ Texas San Antonio, Dept Phys & Astron, San Antonio, TX 78249 USA. EM cl.chen@utsa.edu RI lin, yuan/B-9955-2013; Zhang, Qingyu/O-8472-2015 FU National Science Foundation [NSF-NIRT-0709293]; Natural Science Foundation of China [11329402, 18110225]; Department of Energy [DE-FE0003780]; State of Texas through the Texas Center for Superconductivity at the University of Houston; China Scholarship Council FX This research was partially supported by the National Science Foundation under NSF-NIRT-0709293, the Natural Science Foundation of China under 11329402 and 18110225, the Department of Energy under DE-FE0003780, and the State of Texas through the Texas Center for Superconductivity at the University of Houston. We would like to thank Dr. HD Wu for the dielectric property measurements of the BSTO films. Also, Dr. Ming Liu and Dr. Chunrui Ma would like to acknowledge the support from the "China Scholarship Council" for the program of national study-abroad project for the postgraduates of high level universities at UTSA. NR 30 TC 8 Z9 8 U1 5 U2 81 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD OCT 31 PY 2013 VL 3 AR 3092 DI 10.1038/srep03092 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 243QZ UT WOS:000326333300001 PM 24172706 ER PT J AU Di Leo, RA Marschilok, AC Takeuchi, KJ Takeuchi, ES AF Di Leo, Roberta A. Marschilok, Amy C. Takeuchi, Kenneth J. Takeuchi, Esther S. TI Battery electrolytes based on saturated ring ionic liquids: Physical and electrochemical properties SO ELECTROCHIMICA ACTA LA English DT Article DE Ionic liquid; Lithium battery; Electrolyte; Conductivity; High voltage stability ID LITHIUM BATTERY; CONDUCTIVITY; VISCOSITY; STABILITY; CARBONATE; MIXTURES; CELLS AB Physical and electrochemical properties of mixtures of ionic liquids based on saturated ring systems with carbonate based solvents were investigated. The conductivity and electrochemical stability of two series of ionic liquids based on piperidinium and pyrrolidinium cations with tetrafluoroborate and bis(trifluorosulfonylimide) anions were evaluated. The effects of the ionic liquid cation, substituent chain length of the cation function group, and the anion type on conductivity and electrochemical stability as determined by cyclic voltammetry were studied. The conductivity was influenced by the substituent chain length of the ionic liquid cation and the solvent carbonate type, where higher conductivities were observed with shorter substituent chains and EC versus PC. The saturated ring ionic liquid-carbonate mixtures may show particular promise for implementation as battery electrolytes due to notable high voltage stabilities, where stability >5.5 V was maintained in the presence of lithium salt. This study should promote development of future safe, high voltage lithium ion battery systems. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Di Leo, Roberta A.; Marschilok, Amy C.; Takeuchi, Kenneth J.; Takeuchi, Esther S.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Di Leo, Roberta A.; Marschilok, Amy C.; Takeuchi, Esther S.] SUNY Stony Brook, Dept Mat Sci & Engn, Stony Brook, NY 11794 USA. [Takeuchi, Esther S.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Marschilok, AC (reprint author), SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. EM amy.marschilok@stonybrook.edu; kenneth.takeuchi.1@stonybrook.edu; esther.takeuchi@stonybrook.edu RI Takeuchi, Esther/D-1825-2014; Marschilok, Amy/D-1821-2014 FU Intelligence Community Postdoctoral Research Fellowship Program through Office of the Director of National Intelligence FX This project was supported by a grant from the Intelligence Community Postdoctoral Research Fellowship Program through funding from the Office of the Director of National Intelligence. NR 27 TC 10 Z9 10 U1 1 U2 28 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0013-4686 EI 1873-3859 J9 ELECTROCHIM ACTA JI Electrochim. Acta PD OCT 30 PY 2013 VL 109 BP 27 EP 32 DI 10.1016/j.electacta.2013.07.041 PG 6 WC Electrochemistry SC Electrochemistry GA 266EN UT WOS:000328006300004 ER PT J AU Ren, K McConnell, CA Gan, YX Afjeh, AA Zhang, LH AF Ren, Kai McConnell, Courtney A. Gan, Yong X. Afjeh, Abdollah A. Zhang, Lihua TI Magnetic field enhanced photoelectrochemical response of a nanostructured titanium dioxide anode SO ELECTROCHIMICA ACTA LA English DT Article DE Photoelectrochemical fuel cell; Response to magnet field; Photon excitation; TiO2 nanotube ID TIO2 NANOTUBE ARRAYS; SENSITIZED SOLAR-CELLS; FUEL-CELLS; WASTE-WATER; FABRICATION; ELECTRODE; SEMICONDUCTOR; PERFORMANCE; PROGRESS; SENSORS AB The concept of permanent-magnet photoelectrochemical fuel cell is proposed. The fuel cell contains a TiO2 nanotube anode and a platinum cathode. Water was used as the fuel. The anode has a self-organized high aspect ratio TiO2 nanotube layer made through electrochemical oxidation of Ti. Photocatalysis and permanent magnetic field excitation experiments were performed. The photoelectrochemical responses of the anode to visible (Vis) and ultraviolet (UV) light were studied to examine the magnetic field effect. The open circuit voltages were 0.0564, 0.1625, 0.1898 and 0.376 V. under the excitation of Vis, UV, magnet and magnet + UV, respectively. Current density was measured under different linear potential scanning conditions. It reached a value of 5.23 mA/m(2) just under the excitation of the permanent magnet at a bias voltage of 2 V. Combining the magnetic action and the photovoltaic effect, the titanium dioxide photosensitive anode showed a maximum photocurrent density of 296.05 mA/m(2) at 2 V bias. It is concluded that the absolute value of open circuit voltage (OCV) of the fuel cell due to the exposure to the magnet field is much higher than that due to either UV or Vis light illumination. However, UV light excitation results in higher current density in the measurement. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Ren, Kai; Gan, Yong X.; Afjeh, Abdollah A.] Univ Toledo, Dept Mech Ind & Mfg Engn, Toledo, OH 43606 USA. [McConnell, Courtney A.; Gan, Yong X.] Calif State Polytech Univ Pomona, Dept Mech Engn, Pomona, CA 91768 USA. [Zhang, Lihua] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Gan, YX (reprint author), Calif State Polytech Univ Pomona, Dept Mech Engn, 3801 W Temple Ave, Pomona, CA 91768 USA. EM yxgan@csupomona.edu RI Zhang, Lihua/F-4502-2014 FU US Environmental Protection Agency [SU83529701]; Kellogg Foundation; US Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX This work was supported in part by the US Environmental Protection Agency under Grant Number SU83529701 and the Kellogg Foundation. The electron microscopic research carried out in the Center for Functional Nanomaterials at Brookhaven National Laboratory is supported by the US Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. We appreciate Kathryn Rose for correcting English. NR 30 TC 4 Z9 4 U1 3 U2 26 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0013-4686 EI 1873-3859 J9 ELECTROCHIM ACTA JI Electrochim. Acta PD OCT 30 PY 2013 VL 109 BP 162 EP 167 DI 10.1016/j.electacta.2013.07.081 PG 6 WC Electrochemistry SC Electrochemistry GA 266EN UT WOS:000328006300022 ER PT J AU Xiao, N Li, DY Cui, GF Li, N Tian, D Li, Q Wu, G AF Xiao, Ning Li, Deyu Cui, Guofeng Li, Ning Tian, Dong Li, Qing Wu, Gang TI An effective triblock copolymer as a suppressor for microvia filling via copper electrodeposition SO ELECTROCHIMICA ACTA LA English DT Article DE Microvia filling; Copper electroplating; Suppressor; Triblock copolymer; Adsorbing mechanism ID POLYETHYLENE-GLYCOL; CHLORIDE-ION; PEG; DEPOSITION; SPS; CU; CL; INHIBITION; ADSORPTION; KINETICS AB In this work, an effective suppressor was found in copper electroplating solution for microvia filling. The suppressor is a triblock copolymer comprised of ethylene oxide (EO)-propylene oxide (PO)-ethylene oxide (EO) with a molecular weight of 2900 (EPE 2900). In terms of the obtained filling performance evaluated by observing the obtained cross-sectional views of the microvias after electroplating, the electroplating solution was systematically studied as functions of Cl- concentration, EPE 2900 concentration, and convection conditions. It was found that filling performance was greatly dependent on these key factors. In the developed copper electroplating formulation, EPE 2900 was able to yield sufficient filling performance in a broad Cl- concentration ranging from 3 to 200 ppm, although the optimized value was determined to be about 30 ppm in terms of the best filling performance. During the microvia filling process, Cl- concentration, EPE 2900 concentration, and forced convection would affect each other. Their interactions were studied based on the anchor effect of Cl- on the adsorption of EPE 2900 on Cu substrates. In doing so, extensive electrochemical experiments including galvanostatic measurements, linear sweep voltammetry, electrochemical impedance spectroscopy and cyclic voltammetry were employed to study the adsorption behavior of EPE 2900 on the cathode during both the copper electrodeposition and dissolution processes. An adsorbing mechanism of EPE 2900 on cathode was proposed to elucidate the promotional role in improving the microvia filling performance. (C) 2013 Published by Elsevier Ltd. C1 [Xiao, Ning; Li, Deyu; Li, Ning; Tian, Dong] Harbin Inst Technol, Dept Appl Chem, Harbin 150001, Peoples R China. [Cui, Guofeng] Sun Yat Sen Univ, Sch Chem & Chem Engn, Guangzhou 510275, Guangdong, Peoples R China. [Li, Qing; Wu, Gang] Los Alamos Natl Lab, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA. RP Li, N (reprint author), Harbin Inst Technol, Dept Appl Chem, Harbin 150001, Peoples R China. EM lininghit@263.net; wugang@lanl.gov RI Wu, Gang/E-8536-2010; Li, Qing/G-4502-2011 OI Wu, Gang/0000-0003-4956-5208; Li, Qing/0000-0003-4807-030X FU Highnic Group (China) FX This work was financially supported by Highnic Group (China). NR 34 TC 5 Z9 5 U1 5 U2 40 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0013-4686 EI 1873-3859 J9 ELECTROCHIM ACTA JI Electrochim. Acta PD OCT 30 PY 2013 VL 109 BP 226 EP 232 DI 10.1016/j.electacta.2013.07.127 PG 7 WC Electrochemistry SC Electrochemistry GA 266EN UT WOS:000328006300032 ER PT J AU Komanicky, V Hennessy, DC Iddir, H Zapol, P You, H AF Komanicky, Vladimir Hennessy, Daniel C. Iddir, Hakim Zapol, Peter You, Hoydoo TI Electrocatalytic activity of surface oxides on platinum nanofacets and surfaces SO ELECTROCHIMICA ACTA LA English DT Article DE Platinum catalysts; CO electrooxidation; Bifunctional catalysts; X-rays, DFT ID DENSITY-FUNCTIONAL THEORY; X-RAY-SCATTERING; OXYGEN REDUCTION; PT(100) SURFACE; PT(111); CO; ELECTRODES; OXIDATION; COVERAGE; PT(311) AB We investigated electrochemical behavior of surface oxides of platinum formed by annealing in air. We studied the catalytic activity for CO electrooxidation using electrochemical, X-ray, and DFT methods. We find that all oxidized platinum surfaces are highly active initially for CO electrooxidation reaction in so-called preignition region. While the high activity of the monolayer oxide formed on extended Pt surfaces decreases after the initial CO-oxidation cycle, bilayer oxide formed on nanoscaled facets sustain the high CO electrooxidation activity. DFT calculations show that OH binds, as strongly to bilayer surface oxides as to metallic surface while CO does not, suggesting the bifunctional property of the bilayer oxide surface. Published by Elsevier Ltd. C1 [Komanicky, Vladimir] Safarik Univ, Fac Sci, Kosice 04001, Slovakia. [Hennessy, Daniel C.; Iddir, Hakim; Zapol, Peter; You, Hoydoo] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Komanicky, V (reprint author), Safarik Univ, Fac Sci, Kosice 04001, Slovakia. EM vladimir.komanicky@upjs.sk; hyou@anl.gov RI Zapol, Peter/G-1810-2012; You, Hoydoo/A-6201-2011 OI Zapol, Peter/0000-0003-0570-9169; You, Hoydoo/0000-0003-2996-9483 FU U.S. DOE, BES [DE-AC02-06CH11357]; Slovak grant [VEGA 1/0782/12]; ERDF EU [ITMS 26220120005] FX The work at ANL and the use of the APS were supported by the U.S. DOE, BES, under contract No. DE-AC02-06CH11357 and the work at Safarik University are supported by Slovak grant VEGA 1/0782/12 and ERDF EU grant under contract No. ITMS 26220120005. NR 22 TC 1 Z9 1 U1 1 U2 21 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0013-4686 EI 1873-3859 J9 ELECTROCHIM ACTA JI Electrochim. Acta PD OCT 30 PY 2013 VL 109 BP 440 EP 446 DI 10.1016/j.electacta.2013.07.098 PG 7 WC Electrochemistry SC Electrochemistry GA 266EN UT WOS:000328006300062 ER PT J AU Datta, S Henry, MP Lin, YJ Fracaro, AT Millard, CS Snyder, SW Stiles, RL Shah, J Yuan, JW Wesoloski, L Dorner, RW Carlson, WM AF Datta, Saurav Henry, Michael P. Lin, YuPo J. Fracaro, Anthony T. Millard, Cynthia S. Snyder, Seth W. Stiles, Rebecca L. Shah, Jitendra Yuan, Jianwei Wesoloski, Lisa Dorner, Robert W. Carlson, Wayne M. TI Electrochemical CO2 Capture Using Resin-Wafer Electrodeionization SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID PRESSURE SWING ADSORPTION; CARBON-DIOXIDE CAPTURE; FLUE-GASES; IONIC LIQUID; TECHNOLOGY; SEPARATION; MEMBRANE; WATER; ELECTRODIALYSIS; EFFICIENT AB Energy-efficient capture of CO2 from power-plant flue gas is one of the grand challenges to reduce greenhouse gas (GHG) emissions. Current CO2-capture technologies are limited by parasitic energy loss, inefficient capture, and unfavorable process economics. We present a novel electrochemical method for CO2 capture from coal-fired power-plant flue gas. The method utilizes in-situ electrochemical pH control with a resin wafer electrodeionization (RW-EDI) device that continuously shifts the pH of the process fluid between basic and acidic in sequential chambers (pH swing). This pH swing enables capture of CO2 from flue gas in the basic chamber followed by release (recovery) of the captured CO2 (purified) in the acidic chamber of the same device. The approach is based on the sensitivity of the thermodynamic equilibrium of CO2 hydration/dehydration reactions over a narrow pH range. The method enables simultaneous absorption (capture) of CO2 from flue gas and desorption (release) at atmospheric pressure without heating, vacuum, or consumptive chemical usage. In other words, the method concentrates CO2 from similar to 15% in flue gas to >98% in the recovery stream. To the best of our knowledge, this is the first experimental study focusing on simultaneous capture and release (recovery) of CO2 using an electrochemical method. We describe the method, the role of operating parameters on CO2 recovery, and advancements in process design and engineering for improved efficiency. We report on a method to enhance gas/liquid mixing inside the RW-EDI, which significantly increased CO2 capture rates. We also discuss the importance of using an enzyme/catalyst in enhancing the reaction kinetics. CO2 capture was observed to be a strong function of gas and liquid flow rates and applied electrical field. Up to 80% of the CO2 was captured from a simulated flue gas stream with >98% purity. The results indicate that a narrow pH swing from 8 to 6 (near-neutral pH) could offer a viable pathway for energy-efficient CO2 capture if the reaction kinetics are enhanced. Carbonic anhydrase enzyme enhances the reaction kinetics at near-neutral pH; however, the enzyme lost activity due to the instability at the operating conditions. This observation highlighted the necessity of robust enzymes/catalysts to enhance kinetics of CO2 recovery nearneutral pH. C1 [Datta, Saurav; Henry, Michael P.; Lin, YuPo J.; Fracaro, Anthony T.; Millard, Cynthia S.; Snyder, Seth W.] Argonne Natl Lab, Argonne, IL 60439 USA. [Stiles, Rebecca L.; Shah, Jitendra; Yuan, Jianwei; Wesoloski, Lisa; Dorner, Robert W.; Carlson, Wayne M.] Nalco Co, Air Protect Technol, Naperville, IL 60563 USA. RP Snyder, SW (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. EM seth@anl.gov FU DOE Advanced Research Project Agency-Energy (ARPA-E) [DE-FOA-0000065]; DOE Fossil Energy program [DE-PS26-06NT42829-0]; U.S. Department of Energy Office of Science laboratory [DE-AC02-06CH11357] FX We acknowledge the DOE Advanced Research Project Agency-Energy (ARPA-E) for financial support of this research (Funding Opportunity Number DE-FOA-0000065). The discovery phase of this research was supported by the DOE Fossil Energy program (Funding Opportunity Number DE-PS26-06NT42829-0). The discovery phase work was led by Dr. Michael C. Trachtenberg, Carbozyme, Inc. We thank Dr. Manian Ramesh, Nalco (retired) for his guidance and leadership on assembling the team.; The submitted manuscript was created by UChicago Argonne, LLC, Operator of Argonne National Laboratory ("Argonne"). Argonne, a U.S. Department of Energy Office of Science laboratory, is operated under Contract No. DE-AC02-06CH11357. The U.S. Government retains for itself, and others acting on its behalf, a paid-up nonexclusive, irrevocable worldwide license in said article to reproduce, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, by or on behalf of the Government. NR 53 TC 7 Z9 7 U1 5 U2 55 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 EI 1520-5045 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD OCT 30 PY 2013 VL 52 IS 43 BP 15177 EP 15186 DI 10.1021/ie402538d PG 10 WC Engineering, Chemical SC Engineering GA 245TZ UT WOS:000326488000020 ER PT J AU Carboni, M Abney, CW Taylor-Pashow, KML Vivero-Escoto, JL Lin, WB AF Carboni, Michael Abney, Carter W. Taylor-Pashow, Kathryn M. L. Vivero-Escoto, Juan L. Lin, Wenbin TI Uranium Sorption with Functionalized Mesoporous Carbon Materials SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID SURFACE FUNCTIONALIZATION; HIGHLY EFFICIENT; AQUEOUS-SOLUTION; SEAWATER; RECOVERY; U(VI); ACID; PHOSPHONATE; ADSORPTION; EXTRACTION AB A series of functionalized mesoporous carbon (MC) materials were prepared by covalent grafting with amidoxime, carboxyl, and phosphoryl functional groups and screened for uranium (U) sorption from aqueous media. The MC materials were characterized by nitrogen adsorption measurements and thermogravimetric analysis and investigated for U(VI) extraction from both acidic water (pH 4) and artificial seawater (pH 8.2). Under both conditions, a phosphoric acid-functionalized MC exhibited the highest U(VI) sorption, with a maximum sorption capacity of 97 mg of U(VI)/(g of sorbent) in acidic water and 67 mg of U(VI)/(g of sorbent) in artificial seawater. The effects of pH on U(VI) sorption, sorption kinetics, and sorption isotherms were obtained for the phosphoric acid-functionalized MC. Quantitative U(VI) removal from U(VI)-loaded sorbents was achieved by washing with HCl at concentrations higher than 0.01 M. These results indicate that functionalized MC provides a promising platform for the development of novel sorbents for efficient U(VI) extraction. C1 [Carboni, Michael; Abney, Carter W.; Lin, Wenbin] Univ Chicago, Dept Chem, Chicago, IL 60637 USA. [Taylor-Pashow, Kathryn M. L.] Savannah River Natl Lab, Aiken, SC 29808 USA. [Vivero-Escoto, Juan L.] Univ N Carolina, Dept Chem, Charlotte, NC 28223 USA. RP Lin, WB (reprint author), Univ Chicago, Dept Chem, 929 E 57th St, Chicago, IL 60637 USA. EM wenbinlin@uchicago.edu RI Lin, Wenbin/B-4151-2010; Vivero-Escoto, Juan/I-8015-2014; OI Lin, Wenbin/0000-0001-7035-7759; Abney, Carter/0000-0002-1809-9577 FU DOE Office of Nuclear Energy's Nuclear Energy University Program [20, 120427, 3151] FX This work was supported by the DOE Office of Nuclear Energy's Nuclear Energy University Program (Subcontract 20 #120427, Project #3151). NR 62 TC 29 Z9 29 U1 11 U2 98 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD OCT 30 PY 2013 VL 52 IS 43 BP 15187 EP 15197 DI 10.1021/ie402646r PG 11 WC Engineering, Chemical SC Engineering GA 245TZ UT WOS:000326488000021 ER PT J AU Isacoff, EY Jan, LY Minor, DL AF Isacoff, Ehud Y. Jan, Lily Y. Minor, Daniel L., Jr. TI Conduits of Life's Spark: A Perspective on Ion Channel Research since the Birth of Neuron SO NEURON LA English DT Review ID GATED SODIUM-CHANNEL; SHAKER K+ CHANNEL; NICOTINIC ACETYLCHOLINE-RECEPTOR; VOLTAGE-SENSING DOMAIN; X-RAY-STRUCTURE; HOMEOSTATIC SYNAPTIC PLASTICITY; ACTIVITY-DEPENDENT REGULATION; PROTEIN-COUPLED RECEPTORS; CELL-SURFACE EXPRESSION; EARLY SECRETORY PATHWAY AB Heartbeats, muscle twitches, and lightning-fast thoughts are all manifestations of bioelectricity and rely on the activity of a class of membrane proteins known as ion channels. The basic function of an ion channel can be distilled into, "The hole opens. Ions go through. The hole closes." Studies of the fundamental mechanisms by which this process happens and the consequences of such activity in the setting of excitable cells remains the central focus of much of the field. One might wonder after so many years of detailed poking at such a seemingly simple process, is there anything left to learn? C1 [Isacoff, Ehud Y.] Univ Calif Berkeley, Helen Wills Neurosci Inst, Berkeley, CA 94720 USA. [Isacoff, Ehud Y.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Jan, Lily Y.; Minor, Daniel L., Jr.] Univ Calif San Francisco, Dept Biochem & Biophys, San Francisco, CA 94158 USA. [Jan, Lily Y.] Univ Calif San Francisco, Dept Physiol, San Francisco, CA 94158 USA. [Jan, Lily Y.] Univ Calif San Francisco, Dept Physiol, San Francisco, CA 94158 USA. [Jan, Lily Y.] Univ Calif San Francisco, Howard Hughes Med Inst, San Francisco, CA 94158 USA. [Minor, Daniel L., Jr.] Univ Calif San Francisco, Dept Cellular & Mol Pharmacol, San Francisco, CA 94158 USA. [Minor, Daniel L., Jr.] Univ Calif San Francisco, Cardiovasc Res Inst, San Francisco, CA 94158 USA. [Minor, Daniel L., Jr.] Univ Calif San Francisco, Calif Inst Quantitat Biomed Res, San Francisco, CA 94158 USA. [Isacoff, Ehud Y.; Minor, Daniel L., Jr.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Minor, DL (reprint author), Univ Calif San Francisco, Dept Biochem & Biophys, San Francisco, CA 94158 USA. EM daniel.minor@ucsf.edu FU NIH [R01-HL080050, R01-DC007664, R01-MH093603, U54-GM094625, R01 NS35549, R37MH065334, R01NS069229]; Howard Hughes Medical Institute FX We thank B. Hille and W.A. Catterall for assistance with the figures and K. Brejc for critical comments on the manuscript. We thank Francesco Tombola for helpful discussion. This work was supported by grants to D.L.M. from NIH R01-HL080050, R01-DC007664, R01-MH093603, and U54-GM094625 to E.Y.I. from NIH R01 NS35549, and to L.Y.J. from NIH R37MH065334, R01NS069229, and the Howard Hughes Medical Institute. NR 280 TC 12 Z9 12 U1 2 U2 28 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0896-6273 EI 1097-4199 J9 NEURON JI Neuron PD OCT 30 PY 2013 VL 80 IS 3 BP 658 EP 674 DI 10.1016/j.neuron.2013.10.040 PG 17 WC Neurosciences SC Neurosciences & Neurology GA 247IA UT WOS:000326609900012 PM 24183018 ER PT J AU Pepper, SE Ogden, MD AF Pepper, Sarah E. Ogden, Mark D. TI Perrhenate extraction studies by Cyphos 101-IL; screening for implementation in technetium removal SO SEPARATION AND PURIFICATION TECHNOLOGY LA English DT Article DE Anion exchange; Ionic liquid; Perrhenate; Solvent extraction; Technetium analogue ID HYDROCHLORIC-ACID SOLUTIONS; PHOSPHONIUM IONIC LIQUID; CHLORIDE SOLUTIONS; BIOPOLYMER CAPSULES; PICKLING SOLUTIONS; IRON IONS; RECOVERY; ZINC(II); IL-101; PALLADIUM(II) AB The solvent extraction of rhenium (VII) from chloride solutions by Cyphos 101-IL in toluene has been studied. Distribution values for the extraction of perrhenate are extremely high leading to almost quantitative extraction. From slope analysis, an anion exchange extraction mechanism is proposed, with formation of a ReO4- association with one Cyphos IL-101 cation. The extraction kinetics are fast, with complete equilibration occurring within 60 s. Under identical conditions, distribution coefficients for Cyphos 101-IL are greater than for Aliquat-336. Extraction of the perrhenate anion does not seem to be negatively impacted by common environmental contaminants including iron, sulphate and nitrate at the pH values tested. (C) 2013 Elsevier B.V. All rights reserved. C1 [Pepper, Sarah E.] Idaho Natl Lab, Idaho Falls, ID 83514 USA. [Ogden, Mark D.] ANSTO Minerals, Kirrawee Dc, NSW 2232, Australia. RP Ogden, MD (reprint author), ANSTO Minerals, Locked Bag 2001, Kirrawee Dc, NSW 2232, Australia. EM mark.ogden@ansto.gov.au FU United States Department of Energy, Office of Nuclear Energy, Science and Technology; INL Laboratory Directed Research and Development (LDRD) Program Under DOE-NE Idaho Operations Office [DE-AC07-051D14517] FX This work was supported by the United States Department of Energy, Office of Nuclear Energy, Science and Technology and the INL Laboratory Directed Research and Development (LDRD) Program Under DOE-NE Idaho Operations Office contract DE-AC07-051D14517. The authors also thank Byron White for ICP-MS data analysis. NR 42 TC 4 Z9 4 U1 4 U2 30 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 1383-5866 EI 1873-3794 J9 SEP PURIF TECHNOL JI Sep. Purif. Technol. PD OCT 30 PY 2013 VL 118 BP 847 EP 852 DI 10.1016/j.seppur.2013.08.029 PG 6 WC Engineering, Chemical SC Engineering GA 252HA UT WOS:000326994500104 ER PT J AU Townson, JL Lin, YS Agola, JO Carnes, EC Leong, HS Lewis, JD Haynes, CL Brinker, CJ AF Townson, Jason L. Lin, Yu-Shen Agola, Jacob O. Carnes, Eric C. Leong, Hon S. Lewis, John D. Haynes, Christy L. Brinker, C. Jeffrey TI Re-examining the Size/Charge Paradigm: Differing in Vivo Characteristics of Size- and Charge-Matched Mesoporous Silica Nanoparticles SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID CANCER-CELLS; SYSTEM AB The combination of nanoparticle (NP) size, charge, and surface chemistry (e.g., extent of modification with polyethylene glycol (PEG)) is accepted as a key determinant of NP/cellular interactions. However, the influence of spatial arrangement and accessibility of the charged molecules on the NP surface vis-a-vis the average surface charge (zeta (zeta) potential) is incompletely understood. Here we demonstrate that two types of mesoporous silica nanoparticles (MSNP) that are matched in terms of primary and hydrodynamic particle size, shape, pore structure, colloidal stability, and zeta potential, but differ in surface chemistry, viz, the spatial arrangement and relative exposure of surface amines, have profoundly different interactions with cells and tissues when evaluated in vitro and in vivo. While both particles are similar to 50 nm in diameter, PEGylated, and positively charged (zeta = +40 mV), PEG-PEI (MSNPs modified with exposed poly-amines), but not PEG-NMe3+ (MSNP modified with distributed, obstructed amines) rapidly bind serum proteins, diverse cells types in vitro, and endothelial and white blood cells in vivo (ex ovo chick embryo model). This finding helps elucidate the relative role of surface exposure of charged molecules vs zeta potential in otherwise physicochemically matched MSNP and highlights protein corona neutrality as an important design consideration when synthesizing cationic NPs for biological applications. C1 [Townson, Jason L.; Lin, Yu-Shen; Agola, Jacob O.; Brinker, C. Jeffrey] Univ New Mexico, Ctr Microengn Mat, Albuquerque, NM 87131 USA. [Brinker, C. Jeffrey] Univ New Mexico, Dept Chem Engn, Albuquerque, NM 87131 USA. [Carnes, Eric C.] Sandia Natl Labs, Nanobiol Dept, Albuquerque, NM 87185 USA. [Brinker, C. Jeffrey] Sandia Natl Labs, Self Assembled Mat Dept, Albuquerque, NM 87185 USA. [Leong, Hon S.] London Reg Canc Program, London, England. [Lewis, John D.] Univ Alberta, Dept Oncol, Edmonton, AB, Canada. [Haynes, Christy L.] Univ Minnesota, Dept Chem, Minneapolis, MN 55455 USA. RP Brinker, CJ (reprint author), Univ New Mexico, Ctr Microengn Mat, Albuquerque, NM 87131 USA. EM cjbrink@sandia.gov OI Leong, Hon/0000-0001-7801-1402 FU NIH [UO1 CA151792-01]; Gabrielle's Angel foundation; UNM CNTC; U.S. DOE, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; Sandia National Laboratories' LDRD program; AFOSR [FA 9550-10-1-0054]; NSF; EPA FX We thank Walker Wharton and Katharine Epler for helpful discussions and experimental assistance. This work was funded by NIH Grant UO1 CA151792-01. J.L.T. was supported by a Young Investigators Award from Gabrielle's Angel foundation. Y.S.L. was funded by a fellowship from The UNM CNTC. C.J.B acknowledges additional support from U.S. DOE, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, Sandia National Laboratories' LDRD program, AFOSR grant FA 9550-10-1-0054, NSF and EPA. NR 15 TC 35 Z9 35 U1 2 U2 96 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 EI 1520-5126 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD OCT 30 PY 2013 VL 135 IS 43 BP 16030 EP 16033 DI 10.1021/ja4082414 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA 245TX UT WOS:000326487800017 PM 24107191 ER PT J AU Lees, JP Poireau, V Tisserand, V Grauges, E Palano, A Eigen, G Stugu, B Brown, DN Kerth, LT Kolomensky, YG Lee, MJ Lynch, G Koch, H Schroeder, T Hearty, C Mattison, TS McKenna, JA So, RY Khan, A Blinov, VE Buzykaev, AR Druzhinin, VP Golubev, VB Kravchenko, EA Onuchin, AP Serednyakov, SI Skovpen, YI Solodov, EP Todyshev, KY Yushkov, AN Kirkby, D Lankford, AJ Mandelkern, M Dey, B Gary, JW Long, O Vitug, GM Campagnari, C Sevilla, MF Hong, TM Kovalskyi, D Richman, JD West, CA Eisner, AM Lockman, WS Schumm, BA Seiden, A Chao, DS Cheng, CH Echenard, B Flood, KT Hitlin, DG Ongmongkolkul, P Porter, FC Andreassen, R Huard, Z Meadows, BT Pappenheimer, C Pushpawela, BG Sokoloff, MD Sun, L Bloom, PC Ford, WT Gaz, A Nauenberg, U Smith, JG Wagner, SR Ayad, R Toki, WH Spaan, B Schwierz, R Bernard, D Verderi, M Playfer, S Bettoni, D Bozzi, C Calabrese, R Cibinetto, G Fioravanti, E Garzia, I Luppi, E Piemontese, L Santoro, V Baldini-Ferroli, R Calcaterra, A de Sangro, R Finocchiaro, G Martellotti, S Patteri, P Peruzzi, IM Piccolo, M Rama, M Zallo, A Contri, R Guido, E Lo Vetere, M Monge, MR Passaggio, S Patrignani, C Robutti, E Bhuyan, B Prasad, V Morii, M Adametz, A Uwer, U Lacker, HM Dauncey, PD Mallik, U Chen, C Cochran, J Meyer, WT Prell, S Gritsan, AV Arnaud, N Davier, M Derkach, D Grosdidier, G Le Diberder, F Lutz, AM Malaescu, B Roudeau, P Stocchi, A Wormser, G Lange, DJ Wright, DM Coleman, JP Fry, JR Gabathuler, E Hutchcroft, DE Payne, DJ Touramanis, C Bevan, AJ Di Lodovico, F Sacco, R Cowan, G Bougher, J Brown, DN Davis, CL Denig, AG Fritsch, M Gradl, W Griessinger, K Hafner, A Prencipe, E Schubert, KR Barlow, RJ Lafferty, GD Behn, E Cenci, R Hamilton, B Jawahery, A Roberts, DA Cowan, R Dujmic, D Sciolla, G Cheaib, R Patel, PM Robertson, SH Biassoni, P Neri, N Palombo, F Cremaldi, L Godang, R Sonnek, P Summers, DJ Simard, M Taras, P De Nardo, G Monorchio, D Onorato, G Sciacca, C Martinelli, M Raven, G Jessop, CP LoSecco, JM Honscheid, K Kass, R Brau, J Frey, R Sinev, NB Strom, D Torrence, E Feltresi, E Margoni, M Morandin, M Posocco, M Rotondo, M Simi, G Simonetto, F Stroili, R Akar, S Ben-Haim, E Bomben, M Bonneaud, GR Briand, H Calderini, G Chauveau, J Leruste, P Marchiori, G Ocariz, J Sitt, S Biasini, M Manoni, E Pacetti, S Rossi, A Angelini, C Batignani, G Bettarini, S Carpinelli, M Casarosa, G Cervelli, A Forti, F Giorgi, MA Lusiani, A Oberhof, B Paoloni, E Perez, A Rizzo, G Walsh, JJ Pegna, DL Olsen, J Smith, AJS Faccini, R Ferrarotto, F Ferroni, F Gaspero, M Li Gioi, L Piredda, G Bunger, C Grunberg, O Hartmann, T Leddig, T Voss, C Waldi, R Adye, T Olaiya, EO Wilson, FF Emery, S de Monchenault, GH Vasseur, G Yeche, C Anulli, F Aston, D Bard, DJ Benitez, JF Cartaro, C Convery, MR Dorfan, J Dubois-Felsmann, GP Dunwoodie, W Ebert, M Field, RC Fulsom, BG Gabareen, AM Graham, MT Hast, C Innes, WR Kim, P Kocian, ML Leith, DWGS Lewis, P Lindemann, D Lindquist, B Luitz, S Luth, V Lynch, HL MacFarlane, DB Muller, DR Neal, H Nelson, S Perl, M Pulliam, T Ratcliff, BN Roodman, A Salnikov, AA Schindler, RH Snyder, A Su, D Sullivan, MK Va'vra, J Wagner, AP Wang, WF Wisniewski, WJ Wittgen, M Wright, DH Wulsin, HW Ziegler, V Park, W Purohit, MV White, RM Wilson, JR Randle-Conde, A Sekula, SJ Bellis, M Burchat, PR Miyashita, TS Puccio, EMT Alam, MS Ernst, JA Gorodeisky, R Guttman, N Peimer, DR Soffer, A Spanier, SM Ritchie, JL Ruland, AM Schwitters, RF Wray, BC Izen, JM Lou, XC Bianchi, F De Mori, F Filippi, A Gamba, D Zambito, S Lanceri, L Vitale, L Martinez-Vidal, F Oyanguren, A Villanueva-Perez, P Ahmed, H Albert, J Banerjee, S Bernlochner, FU Choi, HHF King, GJ Kowalewski, R Lewczuk, MJ Lueck, T Nugent, IM Roney, JM Sobie, RJ Tasneem, N Gershon, TJ Harrison, PF Latham, TE Band, HR Dasu, S Pan, Y Prepost, R Wu, SL AF Lees, J. P. Poireau, V. Tisserand, V. Grauges, E. Palano, A. Eigen, G. Stugu, B. Brown, D. N. Kerth, L. T. Kolomensky, Yu. G. Lee, M. J. Lynch, G. Koch, H. Schroeder, T. Hearty, C. Mattison, T. S. McKenna, J. A. So, R. Y. Khan, A. Blinov, V. E. Buzykaev, A. R. Druzhinin, V. P. Golubev, V. B. Kravchenko, E. A. Onuchin, A. P. Serednyakov, S. I. Skovpen, Yu. I. Solodov, E. P. Todyshev, K. Yu. Yushkov, A. N. Kirkby, D. Lankford, A. J. Mandelkern, M. Dey, B. Gary, J. W. Long, O. Vitug, G. M. Campagnari, C. Sevilla, M. Franco Hong, T. M. Kovalskyi, D. Richman, J. D. West, C. A. Eisner, A. M. Lockman, W. S. Schumm, B. A. Seiden, A. Chao, D. S. Cheng, C. H. Echenard, B. Flood, K. T. Hitlin, D. G. Ongmongkolkul, P. Porter, F. C. Andreassen, R. Huard, Z. Meadows, B. T. Pappenheimer, C. Pushpawela, B. G. Sokoloff, M. D. Sun, L. Bloom, P. C. Ford, W. T. Gaz, A. Nauenberg, U. Smith, J. G. Wagner, S. R. Ayad, R. Toki, W. H. Spaan, B. Schwierz, R. Bernard, D. Verderi, M. Playfer, S. Bettoni, D. Bozzi, C. Calabrese, R. Cibinetto, G. Fioravanti, E. Garzia, I. Luppi, E. Piemontese, L. Santoro, V. Baldini-Ferroli, R. Calcaterra, A. de Sangro, R. Finocchiaro, G. Martellotti, S. Patteri, P. Peruzzi, I. M. Piccolo, M. Rama, M. Zallo, A. Contri, R. Guido, E. Lo Vetere, M. Monge, M. R. Passaggio, S. Patrignani, C. Robutti, E. Bhuyan, B. Prasad, V. Morii, M. Adametz, A. Uwer, U. Lacker, H. M. Dauncey, P. D. Mallik, U. Chen, C. Cochran, J. Meyer, W. T. Prell, S. Gritsan, A. V. Arnaud, N. Davier, M. Derkach, D. Grosdidier, G. Le Diberder, F. Lutz, A. M. Malaescu, B. Roudeau, P. Stocchi, A. Wormser, G. Lange, D. J. Wright, D. M. Coleman, J. P. Fry, J. R. Gabathuler, E. Hutchcroft, D. E. Payne, D. J. Touramanis, C. Bevan, A. J. Di Lodovico, F. Sacco, R. Cowan, G. Bougher, J. Brown, D. N. Davis, C. L. Denig, A. G. Fritsch, M. Gradl, W. Griessinger, K. Hafner, A. Prencipe, E. Schubert, K. R. Barlow, R. J. Lafferty, G. D. Behn, E. Cenci, R. Hamilton, B. Jawahery, A. Roberts, D. A. Cowan, R. Dujmic, D. Sciolla, G. Cheaib, R. Patel, P. M. Robertson, S. H. Biassoni, P. Neri, N. Palombo, F. Cremaldi, L. Godang, R. Sonnek, P. Summers, D. J. Simard, M. Taras, P. De Nardo, G. Monorchio, D. Onorato, G. Sciacca, C. Martinelli, M. Raven, G. Jessop, C. P. LoSecco, J. M. Honscheid, K. Kass, R. Brau, J. Frey, R. Sinev, N. B. Strom, D. Torrence, E. Feltresi, E. Margoni, M. Morandin, M. Posocco, M. Rotondo, M. Simi, G. Simonetto, F. Stroili, R. Akar, S. Ben-Haim, E. Bomben, M. Bonneaud, G. R. Briand, H. Calderini, G. Chauveau, J. Leruste, Ph. Marchiori, G. Ocariz, J. Sitt, S. Biasini, M. Manoni, E. Pacetti, S. Rossi, A. Angelini, C. Batignani, G. Bettarini, S. Carpinelli, M. Casarosa, G. Cervelli, A. Forti, F. Giorgi, M. A. Lusiani, A. Oberhof, B. Paoloni, E. Perez, A. Rizzo, G. Walsh, J. J. Pegna, D. Lopes Olsen, J. Smith, A. J. S. Faccini, R. Ferrarotto, F. Ferroni, F. Gaspero, M. Li Gioi, L. Piredda, G. Buenger, C. Gruenberg, O. Hartmann, T. Leddig, T. Voss, C. Waldi, R. Adye, T. Olaiya, E. O. Wilson, F. F. Emery, S. de Monchenault, G. Hamel Vasseur, G. Yeche, Ch. Anulli, F. Aston, D. Bard, D. J. Benitez, J. F. Cartaro, C. Convery, M. R. Dorfan, J. Dubois-Felsmann, G. P. Dunwoodie, W. Ebert, M. Field, R. C. Fulsom, B. G. Gabareen, A. M. Graham, M. T. Hast, C. Innes, W. R. Kim, P. Kocian, M. L. Leith, D. W. G. S. Lewis, P. Lindemann, D. Lindquist, B. Luitz, S. Luth, V. Lynch, H. L. MacFarlane, D. B. Muller, D. R. Neal, H. Nelson, S. Perl, M. Pulliam, T. Ratcliff, B. N. Roodman, A. Salnikov, A. A. Schindler, R. H. Snyder, A. Su, D. Sullivan, M. K. Va'vra, J. Wagner, A. P. Wang, W. F. Wisniewski, W. J. Wittgen, M. Wright, D. H. Wulsin, H. W. Ziegler, V. Park, W. Purohit, M. V. White, R. M. Wilson, J. R. Randle-Conde, A. Sekula, S. J. Bellis, M. Burchat, P. R. Miyashita, T. S. Puccio, E. M. T. Alam, M. S. Ernst, J. A. Gorodeisky, R. Guttman, N. Peimer, D. R. Soffer, A. Spanier, S. M. Ritchie, J. L. Ruland, A. M. Schwitters, R. F. Wray, B. C. Izen, J. M. Lou, X. C. Bianchi, F. De Mori, F. Filippi, A. Gamba, D. Zambito, S. Lanceri, L. Vitale, L. Martinez-Vidal, F. Oyanguren, A. Villanueva-Perez, P. Ahmed, H. Albert, J. Banerjee, Sw. Bernlochner, F. U. Choi, H. H. F. King, G. J. Kowalewski, R. Lewczuk, M. J. Lueck, T. Nugent, I. M. Roney, J. M. Sobie, R. J. Tasneem, N. Gershon, T. J. Harrison, P. F. Latham, T. E. Band, H. R. Dasu, S. Pan, Y. Prepost, R. Wu, S. L. CA BABAR Collaboration TI Measurement of the mass of the D-0 meson SO PHYSICAL REVIEW D LA English DT Article ID BABAR DETECTOR AB We report a measurement of the D-0 meson mass using the decay chain D* (2010) + -> D-0 pi(+) with D-0 -> K-K-K+pi(+). The data were recorded with the BABAR detector at center-of-mass energies at and near the Upsilon(4S) resonance, and correspond to an integrated luminosity of approximately 477 fb(-1). We obtain m(D-0) (1864: 841 +/- 0: 048 +/- 0: 063) MeV, where the quoted errors are statistical and systematic, respectively. 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G. S.; Lewis, P.; Lindemann, D.; Lindquist, B.; Luitz, S.; Luth, V.; Lynch, H. L.; MacFarlane, D. B.; Muller, D. R.; Neal, H.; Nelson, S.; Perl, M.; Pulliam, T.; Ratcliff, B. N.; Roodman, A.; Salnikov, A. A.; Schindler, R. H.; Snyder, A.; Su, D.; Sullivan, M. K.; Va'vra, J.; Wagner, A. P.; Wang, W. F.; Wisniewski, W. J.; Wittgen, M.; Wright, D. H.; Wulsin, H. W.; Ziegler, V.] SLAC Natl Accelerator Lab, Stanford, CA 94309 USA. [Park, W.; Purohit, M. V.; White, R. M.; Wilson, J. R.] Univ S Carolina, Columbia, SC 29208 USA. [Randle-Conde, A.; Sekula, S. J.] So Methodist Univ, Dallas, TX 75275 USA. [Bellis, M.; Burchat, P. R.; Miyashita, T. S.; Puccio, E. M. T.] Stanford Univ, Stanford, CA 94305 USA. [Alam, M. S.; Ernst, J. A.; Gorodeisky, R.] SUNY Albany, Albany, NY 12222 USA. [Guttman, N.; Peimer, D. R.; Soffer, A.] Tel Aviv Univ, Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Spanier, S. M.] Univ Tennessee, Knoxville, TN 37996 USA. [Ritchie, J. L.; Ruland, A. M.; Schwitters, R. F.; Wray, B. C.] Univ Texas Austin, Austin, TX 78712 USA. [Izen, J. M.; Lou, X. C.] Univ Texas Dallas, Richardson, TX 75083 USA. [Bianchi, F.; De Mori, F.; Filippi, A.; Gamba, D.; Zambito, S.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Bianchi, F.; De Mori, F.; Gamba, D.; Zambito, S.] Univ Turin, Dipartimento Fis, I-10125 Turin, Italy. [Lanceri, L.; Vitale, L.] Ist Nazl Fis Nucl, Sez Trieste, I-34127 Trieste, Italy. [Lanceri, L.; Vitale, L.] Univ Trieste, Dipartmento Fis, I-34127 Trieste, Italy. [Martinez-Vidal, F.; Oyanguren, A.; Villanueva-Perez, P.] Univ Valencia, CSIC, IFIC, E-46071 Valencia, Spain. [Ahmed, H.; Albert, J.; Banerjee, Sw.; Bernlochner, F. U.; Choi, H. H. F.; King, G. J.; Kowalewski, R.; Lewczuk, M. J.; Lueck, T.; Nugent, I. M.; Roney, J. M.; Sobie, R. J.; Tasneem, N.] Univ Victoria, Victoria, BC V8W 3P6, Canada. [Gershon, T. J.; Harrison, P. F.; Latham, T. E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Band, H. R.; Dasu, S.; Pan, Y.; Prepost, R.; Wu, S. L.] Univ Wisconsin, Madison, WI 53706 USA. [Anulli, F.] Univ Sassari, I-07100 Sassari, Italy. RP Lees, JP (reprint author), Univ Savoie, CNRS, IN2P3, Lab Annecy Le Vieux Phys Particules LAPP, F-74941 Annecy Le Vieux, France. RI Forti, Francesco/H-3035-2011; Oyanguren, Arantza/K-6454-2014; Luppi, Eleonora/A-4902-2015; White, Ryan/E-2979-2015; Kravchenko, Evgeniy/F-5457-2015; Calabrese, Roberto/G-4405-2015; Martinez Vidal, F*/L-7563-2014; Kolomensky, Yury/I-3510-2015; Lo Vetere, Maurizio/J-5049-2012; Lusiani, Alberto/N-2976-2015; Patrignani, Claudia/C-5223-2009; Monge, Maria Roberta/G-9127-2012; Rizzo, Giuliana/A-8516-2015; Morandin, Mauro/A-3308-2016; Lusiani, Alberto/A-3329-2016; Di Lodovico, Francesca/L-9109-2016; Calcaterra, Alessandro/P-5260-2015; Frey, Raymond/E-2830-2016; OI Forti, Francesco/0000-0001-6535-7965; Oyanguren, Arantza/0000-0002-8240-7300; Luppi, Eleonora/0000-0002-1072-5633; White, Ryan/0000-0003-3589-5900; Calabrese, Roberto/0000-0002-1354-5400; Martinez Vidal, F*/0000-0001-6841-6035; Kolomensky, Yury/0000-0001-8496-9975; Lo Vetere, Maurizio/0000-0002-6520-4480; Lusiani, Alberto/0000-0002-6876-3288; Patrignani, Claudia/0000-0002-5882-1747; Monge, Maria Roberta/0000-0003-1633-3195; Cibinetto, Gianluigi/0000-0002-3491-6231; Pacetti, Simone/0000-0002-6385-3508; Rizzo, Giuliana/0000-0003-1788-2866; Faccini, Riccardo/0000-0003-2613-5141; Bellis, Matthew/0000-0002-6353-6043; Morandin, Mauro/0000-0003-4708-4240; Lusiani, Alberto/0000-0002-6876-3288; Di Lodovico, Francesca/0000-0003-3952-2175; Calcaterra, Alessandro/0000-0003-2670-4826; Frey, Raymond/0000-0003-0341-2636; Martinelli, Maurizio/0000-0003-4792-9178; Lanceri, Livio/0000-0001-8220-3095; Sciacca, Crisostomo/0000-0002-8412-4072; Ebert, Marcus/0000-0002-3014-1512; Paoloni, Eugenio/0000-0001-5969-8712; Bettarini, Stefano/0000-0001-7742-2998 FU U.S. Department of Energy and National Science Foundation,; Natural Sciences and Engineering Research Council (Canada); Commissariat a l'Energie Atomique and Institut National de Physique Nucle aire et de Physique des Particules (France); Bundesministerium fur Bildung und Forschung and Deutsche Forschungsgemeinschaft (Germany); Istituto Nazionale di Fisica Nucleare (Italy); Foundation for Fundamental Research on Matter (The Netherlands); Research Council of Norway; Ministry of Education and Science of the Russian Federation; Ministerio de Ciencia e Innovacion (Spain); Science and Technology Facilities Council (United Kingdom); Marie-Curie IEF program (European Union); WISE (Women in Science and Engineering) fellowship; A. P. Sloan Foundation (USA) FX We are grateful for the extraordinary contributions of our PEP- II colleagues in achieving the excellent luminosity and machine conditions that have made this work possible. The success of this project also relies critically on the expertise and dedication of the computing organizations that support BABAR. The collaborating institutions wish to thank SLAC for its support and the kind hospitality extended to them. This work is supported by the U.S. Department of Energy and National Science Foundation, the Natural Sciences and Engineering Research Council (Canada), the Commissariat a l'Energie Atomique and Institut National de Physique Nucle aire et de Physique des Particules (France), the Bundesministerium fur Bildung und Forschung and Deutsche Forschungsgemeinschaft (Germany), the Istituto Nazionale di Fisica Nucleare (Italy), the Foundation for Fundamental Research on Matter (The Netherlands), the Research Council of Norway, the Ministry of Education and Science of the Russian Federation, Ministerio de Ciencia e Innovacion (Spain), and the Science and Technology Facilities Council (United Kingdom). Individuals have received support from the Marie-Curie IEF program (European Union) and the A. P. Sloan Foundation (USA). The University of Cincinnati is gratefully acknowledged for its support of this research through a WISE (Women in Science and Engineering) fellowship to C. Pappenheimer. NR 16 TC 6 Z9 6 U1 1 U2 22 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD OCT 30 PY 2013 VL 88 IS 7 AR 071104 DI 10.1103/PhysRevD.88.071104 PG 7 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 242WQ UT WOS:000326276100001 ER PT J AU Aaltonen, T Amerio, S Amidei, D Anastassov, A Annovi, A Antos, J Apollinari, G Appel, JA Arisawa, T Artikov, A Asaadi, J Ashmanskas, W Auerbach, B Aurisano, A Azfar, F Badgett, W Bae, T Barbaro-Galtieri, A Barnes, VE Barnett, BA Barria, P Bartos, P Bauce, M Bedeschi, F Behari, S Bellettini, G Bellinger, J Benjamin, D Beretvas, A Bhatti, A Bland, KR Blumenfeld, B Bocci, A Bodek, A Bortoletto, D Boudreau, J Boveia, A Brigliadori, L Bromberg, C Brucken, E Budagov, J Budd, HS Burkett, K Busetto, G Bussey, P Butti, P Buzatu, A Calamba, A Camarda, S Campanelli, M Canelli, F Carls, B Carlsmith, D Carosi, R Carrillo, S Casal, B Casarsa, M Castro, A Catastini, P Cauz, D Cavaliere, V Cavalli-Sforza, M Cerri, A Cerrito, L Chen, YC Chertok, M Chiarelli, G Chlachidze, G Cho, K Chokheli, D Clark, A Clarke, C Convery, ME Conway, J Corbo, M Cordelli, M Cox, CA Cox, DJ Cremonesi, M Cruz, D Cuevas, J Culbertson, R d'Ascenzo, N Datta, M De Barbaro, P Demortier, L Deninno, M D'Errico, M Devoto, F Di Canto, A Di Ruzza, B Dittmann, JR Donati, S D'Onofrio, M Dorigo, M Driutti, A Ebina, K Edgar, R Elagin, A Erbacher, R Errede, S Esham, B Farrington, S Ramos, JPF Field, R Flanagan, G Forrest, R Franklin, M Freeman, JC Frisch, H Funakoshi, Y Galloni, C Garfinkel, AF Garosi, P Gerberich, H Gerchtein, E Giagua, S Giakoumopoulou, V Gibson, K Ginsburg, CM Giokaris, N Giromini, P Giurgiu, G Glagolev, V Glenzinski, D Gold, M Goldin, D Golossanov, A Gomez, G Gomez-Ceballos, G Goncharov, M Lopez, OG Gorelov, I Goshaw, AT Goulianos, K Gramellinia, E Grinstein, S Grosso-Pilcher, C Group, RC da Costa, JG Hahn, SR Han, JY Happacher, F Hara, K Hare, M Harr, RF Harrington-Taber, T Hatakeyama, K Hays, C Heinrich, J Herndon, M Hocker, A Hong, Z Hopkins, W Hou, S Hughes, RE Husemann, U Hussein, M Huston, J Introzzi, G Iori, M Ivanov, A James, E Jang, D Jayatilaka, B Jeon, EJ Jindariani, S Jones, M Joo, KK Jun, SY Junk, TR Kambeitz, M Kamon, T Karchin, PE Kasmi, A Kato, Y Ketchum, W Keung, J Kilminster, B Kim, DH Kim, HS Kim, JE Kim, MJ Kim, SH Kim, SB Kim, YJ Kim, YK Kimura, N Kirby, M Knoepfel, K Kondo, K Kong, DJ Konigsberg, J Kotwal, AV Kreps, M Kroll, J Kruse, M Kuhr, T Kurata, M Laasanen, AT Lammel, S Lancaster, M Lannon, K Latino, G Lee, HS Lee, JS Leo, S Leone, S Lewis, JD Limosani, A Lipeles, E Lister, A Liu, H Liu, Q Liu, T Lockwitz, S Loginov, A Lucchesi, D Luca, A Lueck, J Lujan, P Lukens, P Lungu, G Lys, J Lysak, R Madrak, R Maestro, P Malik, S Manca, G Manousakis-Katsikakis, A Marchese, L Margaroli, F Marino, P Martinez, M Matera, K Mattson, ME Mazzacane, A Mazzanti, P McNulty, R Mehta, A Mehtala, P Mesropian, C Miao, T Mietlicki, D Mitra, A Miyake, H Moed, S Moggi, N Moon, CS Moore, R Morello, MJ Mukherjee, A Muller, T Murat, P Mussini, M Nachtman, J Nagai, Y Naganoma, J Nakano, I Napier, A Nett, J Neu, C Nigmanov, T Nodulman, L Noh, SY Norniella, O Oakes, L Oh, SH Oh, YD Oksuzian, I Okusawa, T Orava, R Ortolan, L Pagliaronea, C Palencia, E Palni, P Papadimitriou, V Parker, W Pauletta, G Paulini, M Paus, C Phillips, TJ Piacentino, G Pianori, E Pilot, J Pitts, K Plager, C Pondrom, L Poprocki, S Potamianos, K Pranko, A Prokoshin, F Ptohos, F Punzi, G Ranjan, N Fernandez, IR Renton, P Rescigno, M Rimondi, F Ristori, L Robson, A Rodriguez, T Rolli, S Ronzani, M Roser, R Rosner, JL Ruffini, F Ruiz, A Russ, J Rusu, V Sakumoto, WK Sakurai, Y Santi, L Sato, K Saveliev, V Savoy-Navarro, A Schlabach, P Schmidt, EE Schwarz, T Scodellaro, L Scuri, F Seidel, S Seiya, Y Semenov, A Sforza, F Shalhout, SZ Shears, T Shepard, PF Shimojima, M Shochet, M Shreyber-Tecker, I Simonenko, A Sliwa, K Smith, JR Snider, FD Song, H Sorin, V Denis, RS Stancari, M Stentz, D Strologas, J Sudo, Y Sukhanov, A Suslov, I Takemasa, K Takeuchi, Y Tang, J Tecchio, M Teng, PK Thom, J Thomson, E Thukral, V Toback, D Tokar, S Tollefson, K Tomura, T Tonelli, D Torre, S Torretta, D Totaro, P Trovato, M Ukegawa, F Uozumi, S Vazquez, F Velev, G Vellidis, C Vernieri, C Vidal, M Vilar, R Vizan, J Vogel, M Volpi, G Wagner, P Wallny, R Wang, SM Waters, D Wester, WC Whiteson, D Wicklund, AB Wilbur, S Williams, HH Wilson, JS Wilson, P Winer, BL Wittich, P Wolbers, S Wolfe, H Wright, T Wu, X Wu, Z Yamamoto, K Yamato, D Yang, T Yang, UK Yang, YC Yao, WM Yeh, GP Yi, K Yoh, J Yorita, K Yoshida, T Yu, GB Yu, I Zanetti, AM Zeng, Y Zhou, C Zucchelli, S AF Aaltonen, T. Amerio, S. Amidei, D. Anastassov, A. Annovi, A. Antos, J. Apollinari, G. Appel, J. A. Arisawa, T. Artikov, A. Asaadi, J. Ashmanskas, W. Auerbach, B. Aurisano, A. Azfar, F. Badgett, W. Bae, T. Barbaro-Galtieri, A. Barnes, V. E. Barnett, B. A. Barria, P. Bartos, P. Bauce, M. Bedeschi, F. Behari, S. Bellettini, G. Bellinger, J. Benjamin, D. Beretvas, A. Bhatti, A. Bland, K. R. Blumenfeld, B. Bocci, A. Bodek, A. Bortoletto, D. Boudreau, J. Boveia, A. Brigliadori, L. Bromberg, C. Brucken, E. Budagov, J. Budd, H. S. Burkett, K. Busetto, G. Bussey, P. Butti, P. Buzatu, A. Calamba, A. Camarda, S. Campanelli, M. Canelli, F. Carls, B. Carlsmith, D. Carosi, R. Carrillo, S. Casal, B. Casarsa, M. Castro, A. Catastini, P. Cauz, D. Cavaliere, V. Cavalli-Sforza, M. Cerri, A. Cerrito, L. Chen, Y. C. Chertok, M. Chiarelli, G. Chlachidze, G. Cho, K. Chokheli, D. Clark, A. Clarke, C. Convery, M. E. Conway, J. Corbo, M. Cordelli, M. Cox, C. A. Cox, D. J. Cremonesi, M. Cruz, D. Cuevas, J. 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CA CDF Collaboration TI Measurement of the Differential Cross Section d sigma/d(cos theta(t)) for Top-Quark Pair Production in p(p)over-bar Collisions at root s = 1.96 TeV SO PHYSICAL REVIEW LETTERS LA English DT Article ID CHARGE ASYMMETRY; GENERAL-THEORY; DETECTOR; PHYSICS AB We report a measurement of the differential cross section d sigma = d(cos theta(t)) for top-quark pair production as a function of the top-quark production angle in proton-antiproton collisions at root s = 1.96 TeV. This measurement is performed using data collected with the CDF II detector at the Tevatron, corresponding to an integrated luminosity of 9.4 fb(-1). We employ the Legendre polynomials to characterize the shape of the differential cross section at the parton level. The observed Legendre coefficients are in good agreement with the prediction of the next-to-leading-order standard- model calculation, with the exception of an excess linear-term coefficient a(1) = 0.40 +/- 0.12, compared to the standard-model prediction of a(1) = 0.15(-0.03)(+0.07) C1 [Chen, Y. C.; Hou, S.; Mitra, A.; Teng, P. K.; Wang, S. M.] Acad Sinica, Inst Phys, Taipei 11529, Taiwan. [Auerbach, B.; Nodulman, L.; Wicklund, A. B.] Argonne Natl Lab, Argonne, IL 60439 USA. [Giakoumopoulou, V.; Giokaris, N.; Manousakis-Katsikakis, A.] Univ Athens, GR-15771 Athens, Greece. [Camarda, S.; Cavalli-Sforza, M.; Grinstein, S.; Martinez, M.; Ortolan, L.; Sorin, V.] Univ Autonoma Barcelona, Inst Fis Altes Energies, ICREA, E-08193 Bellaterra, Barcelona, Spain. [Bland, K. R.; Dittmann, J. R.; Hatakeyama, K.; Kasmi, A.; Wu, Z.] Baylor Univ, Waco, TX 76798 USA. [Gramellinia, E.; Marchese, L.; Mazzanti, P.; Moggi, N.; Mussini, M.; Rimondi, F.; Zucchelli, S.] Ist Nazl Fis Nucl, I-40127 Bologna, Italy. [Mussini, M.; Zucchelli, S.] Univ Bologna, I-40127 Bologna, Italy. [Chertok, M.; Conway, J.; Cox, C. A.; Cox, D. J.; Erbacher, R.; Forrest, R.; Ivanov, A.; Pilot, J.; Shalhout, S. Z.; Smith, J. R.; Wilbur, S.] Univ Calif Davis, Davis, CA 95616 USA. [Plager, C.] Univ Calif Los Angeles, Los Angeles, CA 90024 USA. [Casal, B.; Cuevas, J.; Gomez, G.; Palencia, E.; Ruiz, A.; Scodellaro, L.; Vilar, R.; Vizan, J.] CSIC Univ Cantabria, Inst Fis Cantabria, Santander 39005, Spain. [Calamba, A.; Jang, D.; Jun, S. Y.; Paulini, M.; Russ, J.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Boveia, A.; Canelli, F.; Frisch, H.; Grosso-Pilcher, C.; Ketchum, W.; Kim, Y. K.; Rosner, J. L.; Shochet, M.; Tang, J.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Antos, J.; Bartos, P.; Lysak, R.; Tokar, S.] Comenius Univ, Bratislava 84248, Slovakia. 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C.; Yu, I.] Kyungpook Natl Univ, Ctr High Energy Phys, Taegu 702701, South Korea. [Bae, T.; Cho, K.; Jeon, E. J.; Joo, K. K.; Kamon, T.; Kim, D. H.; Kim, H. S.; Kim, J. E.; Kim, S. B.; Kim, Y. J.; Kong, D. J.; Lee, H. S.; Lee, J. S.; Noh, S. Y.; Oh, Y. D.; Uozumi, S.; Yang, U. K.; Yang, Y. C.; Yu, I.] Seoul Natl Univ, Seoul 151742, South Korea. [Bae, T.; Cho, K.; Jeon, E. J.; Joo, K. K.; Kamon, T.; Kim, D. H.; Kim, H. S.; Kim, J. E.; Kim, S. B.; Kim, Y. J.; Kong, D. J.; Lee, H. S.; Lee, J. S.; Noh, S. Y.; Oh, Y. D.; Uozumi, S.; Yang, U. K.; Yang, Y. C.; Yu, I.] Sungkyunkwan Univ, Suwon 440746, South Korea. [Bae, T.; Cho, K.; Jeon, E. J.; Joo, K. K.; Kamon, T.; Kim, D. H.; Kim, H. S.; Kim, J. E.; Kim, S. B.; Kim, Y. J.; Kong, D. J.; Lee, H. S.; Lee, J. S.; Noh, S. Y.; Oh, Y. D.; Uozumi, S.; Yang, U. K.; Yang, Y. C.; Yu, I.] Korea Inst Sci & Technol Informat, Taejon 305806, South Korea. [Bae, T.; Cho, K.; Jeon, E. J.; Joo, K. K.; Kamon, T.; Kim, D. H.; Kim, H. S.; Kim, J. E.; Kim, S. 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[Campanelli, M.; Cerrito, L.; Lancaster, M.; Waters, D.] UCL, London WC1E 6BT, England. [Ramos, J. P. Fernandez; Lopez, O. Gonzalez; Fernandez, I. Redondo] CIEMAT, E-28040 Madrid, Spain. [Gomez-Ceballos, G.; Goncharov, M.; Paus, C.] MIT, Cambridge, MA 02139 USA. [Amidei, D.; Edgar, R.; Mietlicki, D.; Schwarz, T.; Tecchio, M.; Wilson, J. S.; Wright, T.] Univ Michigan, Ann Arbor, MI 48109 USA. [Bromberg, C.; Hussein, M.; Huston, J.; Tollefson, K.] Michigan State Univ, E Lansing, MI 48824 USA. [Shreyber-Tecker, I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Gold, M.; Gorelov, I.; Palni, P.; Seidel, S.; Strologas, J.; Vogel, M.] Univ New Mexico, Albuquerque, NM 87131 USA. [Hughes, R. E.; Lannon, K.; Winer, B. L.; Wolfe, H.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Okayama 7008530, Japan. [Kato, Y.; Okusawa, T.; Seiya, Y.; Yamamoto, K.; Yamato, D.; Yoshida, T.] Osaka City Univ, Osaka 5588585, Japan. 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[Bellettini, G.; Butti, P.; Di Canto, A.; Donati, S.; Galloni, C.; Punzi, G.; Ronzani, M.; Sforza, F.] Univ Pisa, I-56127 Pisa, Italy. [Barria, P.; Garosi, P.; Latino, G.; Maestro, P.; Ruffini, F.] Univ Siena, I-27100 Pavia, Italy. [Marino, P.; Morello, M. J.; Trovato, M.; Vernieri, C.] Scuola Normale Super Pisa, I-56127 Pisa, Italy. [Introzzi, G.] Ist Nazl Fis Nucl, I-27100 Pavia, Italy. [Introzzi, G.] Univ Pavia, I-27100 Pavia, Italy. [Boudreau, J.; Gibson, K.; Nigmanov, T.; Shepard, P. F.; Song, H.] Univ Pittsburgh, Pittsburgh, PA 15260 USA. [Barnes, V. E.; Bortoletto, D.; Garfinkel, A. F.; Jones, M.; Laasanen, A. T.; Liu, Q.; Ranjan, N.; Vidal, M.] Purdue Univ, W Lafayette, IN 47907 USA. [Bodek, A.; Budd, H. S.; De Barbaro, P.; Han, J. Y.; Sakumoto, W. K.] Univ Rochester, Rochester, NY 14627 USA. [Bhatti, A.; Demortier, L.; Goulianos, K.; Lungu, G.; Malik, S.; Mesropian, C.] Rockefeller Univ, New York, NY 10065 USA. [Giagua, S.; Iori, M.; Margaroli, F.; Rescigno, M.] Ist Nazl Fis Nucl, Sez Roma 1, I-00185 Rome, Italy. [Iori, M.] Univ Roma La Sapienza, I-00185 Rome, Italy. [Asaadi, J.; Aurisano, A.; Cruz, D.; Elagin, A.; Goldin, D.; Hong, Z.; Kamon, T.; Nett, J.; Thukral, V.; Toback, D.] Texas A&M Univ, Mitchell Inst Fundamental Phys & Astron, College Stn, TX 77843 USA. [Casarsa, M.; Cauz, D.; Dorigo, M.; Driutti, A.; Pagliaronea, C.; Pauletta, G.; Santi, L.; Zanetti, A. M.] Ist Nazl Fis Nucl, I-34127 Trieste, Italy. [Cauz, D.; Dorigo, M.; Driutti, A.; Pauletta, G.; Santi, L.] Grp Collegato Udine, I-33100 Udine, Italy. [Cauz, D.; Driutti, A.; Pauletta, G.; Santi, L.] Univ Udine, I-33100 Udine, Italy. Univ Trieste, I-34127 Trieste, Italy. [Hara, K.; Kim, S. H.; Kurata, M.; Miyake, H.; Nagai, Y.; Sato, K.; Shimojima, M.; Sudo, Y.; Takemasa, K.; Takeuchi, Y.; Tomura, T.; Ukegawa, F.] Univ Tsukuba, Tsukuba, Ibaraki 305, Japan. [Hare, M.; Napier, A.; Rolli, S.; Sliwa, K.] Tufts Univ, Medford, MA 02155 USA. [Group, R. C.; Liu, H.; Neu, C.; Oksuzian, I.] Univ Virginia, Charlottesville, VA 22906 USA. [Arisawa, T.; Ebina, K.; Funakoshi, Y.; Kimura, N.; Kondo, K.; Naganoma, J.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo 169, Japan. [Clarke, C.; Harr, R. F.; Karchin, P. E.; Mattson, M. E.] Wayne State Univ, Detroit, MI 48201 USA. [Bellinger, J.; Carlsmith, D.; Herndon, M.; Parker, W.; Pondrom, L.] Univ Wisconsin, Madison, WI 53706 USA. [Husemann, U.; Lockwitz, S.; Loginov, A.] Yale Univ, New Haven, CT 06520 USA. RP Aaltonen, T (reprint author), Univ Helsinki, Div High Energy Phys, Dept Phys, FIN-00014 Helsinki, Finland. RI Introzzi, Gianluca/K-2497-2015; Piacentino, Giovanni/K-3269-2015; Marino, Pietro/N-7030-2015; song, hao/I-2782-2012; Gorelov, Igor/J-9010-2015; Prokoshin, Fedor/E-2795-2012; Chiarelli, Giorgio/E-8953-2012; Kim, Soo-Bong/B-7061-2014; Robson, Aidan/G-1087-2011; maestro, paolo/E-3280-2010; Lysak, Roman/H-2995-2014; Moon, Chang-Seong/J-3619-2014; Scodellaro, Luca/K-9091-2014; Punzi, Giovanni/J-4947-2012; Grinstein, Sebastian/N-3988-2014; Paulini, Manfred/N-7794-2014; Russ, James/P-3092-2014; vilar, rocio/P-8480-2014; Cavalli-Sforza, Matteo/H-7102-2015 OI Introzzi, Gianluca/0000-0002-1314-2580; Piacentino, Giovanni/0000-0001-9884-2924; Marino, Pietro/0000-0003-0554-3066; song, hao/0000-0002-3134-782X; Gorelov, Igor/0000-0001-5570-0133; Prokoshin, Fedor/0000-0001-6389-5399; Chiarelli, Giorgio/0000-0001-9851-4816; maestro, paolo/0000-0002-4193-1288; Moon, Chang-Seong/0000-0001-8229-7829; Scodellaro, Luca/0000-0002-4974-8330; Punzi, Giovanni/0000-0002-8346-9052; Grinstein, Sebastian/0000-0002-6460-8694; Paulini, Manfred/0000-0002-6714-5787; Russ, James/0000-0001-9856-9155; FU U.S. Department of Energy and National Science Foundation; Italian Istituto Nazionale di Fisica Nucleare; Ministry of Education, Culture, Sports, Science, and Technology of Japan; Natural Sciences and Engineering Research Council of Canada; National Science Council of the Republic of China; Swiss National Science Foundation; A. P. Sloan Foundation; Bundesministerium fur Bildung und Forschung, Germany; Korean World Class University Program; National Research Foundation of Korea; Science and Technology Facilities Council; Royal Society, U. K.; Russian Foundation for Basic Research; Ministerio de Ciencia e Innovacion and Programa Consolider-Ingenio, Spain; Slovak RD Agency; Academy of Finland; Australian Research Council (ARC); EU Community Marie Curie Fellowship [302103] FX We thank T. Tait, S. Jung, W. Bernreuther, and Z.-G. Si for their assistance in preparing the theoretical models and calculations used in this Letter, and T. Rizzo for helpful conversations. We also thank the development teams of SCIPY, PYTABLES, MATPLOTLIB, and IPYTHON for their useful tools [31]. We thank the Fermilab staff and the technical staffs of the participating institutions for their vital contributions. This work was supported by the U.S. Department of Energy and National Science Foundation; the Italian Istituto Nazionale di Fisica Nucleare; the Ministry of Education, Culture, Sports, Science, and Technology of Japan; the Natural Sciences and Engineering Research Council of Canada; the National Science Council of the Republic of China; the Swiss National Science Foundation; the A. P. Sloan Foundation; the Bundesministerium fur Bildung und Forschung, Germany; the Korean World Class University Program and the National Research Foundation of Korea; the Science and Technology Facilities Council and the Royal Society, U. K.; the Russian Foundation for Basic Research; the Ministerio de Ciencia e Innovacion and Programa Consolider-Ingenio 2010, Spain; the Slovak R&D Agency; the Academy of Finland; the Australian Research Council (ARC); and the EU Community Marie Curie Fellowship Contract No. 302103. NR 32 TC 18 Z9 18 U1 2 U2 22 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 30 PY 2013 VL 111 IS 18 AR 182002 DI 10.1103/PhysRevLett.111.182002 PG 8 WC Physics, Multidisciplinary SC Physics GA 242XP UT WOS:000326279400004 PM 24237509 ER PT J AU Gopalakrishnan, S Martin, I Demler, EA AF Gopalakrishnan, Sarang Martin, Ivar Demler, Eugene A. TI Quantum Quasicrystals of Spin-Orbit-Coupled Dipolar Bosons SO PHYSICAL REVIEW LETTERS LA English DT Article ID ORDER; SUPERCONDUCTORS; SYMMETRY; PHASE; FIELD AB We study quasi-two-dimensional dipolar Bose gases in which the bosons experience a Rashba spin-orbit coupling. We show that the degenerate dispersion minimum due to the spin-orbit coupling, combined with the long-range dipolar interaction, can stabilize a number of quantum crystalline and quasicrystalline ground states. Coupling the bosons to a fermionic species can further stabilize these phases. We estimate that the crystalline and quasicrystalline phases should be detectable in realistic dipolar condensates, e.g., dysprosium, and discuss their symmetries and excitations. C1 [Gopalakrishnan, Sarang; Demler, Eugene A.] Harvard Univ, Dept Phys, Cambridge, MA 02138 USA. [Martin, Ivar] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Gopalakrishnan, S (reprint author), Harvard Univ, Dept Phys, Cambridge, MA 02138 USA. FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC020-6CH11357]; Harvard-MIT CUA; DARPA OLE program; AFOSR MURI on Ultracold Molecules; ARO-MURI on Atomtronics FX We are grateful to A. Rosch, B. Lev, R. Wilson, and M. Knap for helpful discussions. S. G. was supported in part by the Harvard Quantum Optics Center. Work performed at Argonne National Laboratory (by I. M.) is supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC020-6CH11357. E. A. D. acknowledges support from Harvard-MIT CUA, the DARPA OLE program, AFOSR MURI on Ultracold Molecules, and ARO-MURI on Atomtronics. NR 53 TC 24 Z9 24 U1 2 U2 23 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 30 PY 2013 VL 111 IS 18 AR 185304 DI 10.1103/PhysRevLett.111.185304 PG 5 WC Physics, Multidisciplinary SC Physics GA 242XP UT WOS:000326279400008 ER PT J AU Fan, ZS Jastrow, JD Liang, C Matamala, R Miller, RM AF Fan, Zhaosheng Jastrow, Julie D. Liang, Chao Matamala, Roser Miller, Raymond Michael TI Priming Effects in Boreal Black Spruce Forest Soils: Quantitative Evaluation and Sensitivity Analysis SO PLOS ONE LA English DT Article ID DISSOLVED ORGANIC-CARBON; INTERIOR ALASKA; HYDRAULIC CONDUCTIVITY; MATTER; DECOMPOSITION; TURNOVER; RESPIRATION; MECHANISMS; PEATLANDS; TRANSPORT AB Laboratory studies show that introduction of fresh and easily decomposable organic carbon (OC) into soil-water systems can stimulate the decomposition of soil OC (SOC) via priming effects in temperate forests, shrublands, grasslands, and agro-ecosystems. However, priming effects are still not well understood in the field setting for temperate ecosystems and virtually nothing is known about priming effects (e. g., existence, frequency, and magnitude) in boreal ecosystems. In this study, a coupled dissolved OC (DOC) transport and microbial biomass dynamics model was developed to simultaneously simulate co-occurring hydrological, physical, and biological processes and their interactions in soil pore-water systems. The developed model was then used to examine the importance of priming effects in two black spruce forest soils, with and without underlying permafrost. Our simulations showed that priming effects were strongly controlled by the frequency and intensity of DOC input, with greater priming effects associated with greater DOC inputs. Sensitivity analyses indicated that priming effects were most sensitive to variations in the quality of SOC, followed by variations in microbial biomass dynamics (i.e., microbial death and maintenance respiration), highlighting the urgent need to better discern these key parameters in future experiments and to consider these dynamics in existing ecosystem models. Water movement carries DOC to deep soil layers that have high SOC stocks in boreal soils. Thus, greater priming effects were predicted for the site with favorable water movement than for the site with limited water flow, suggesting that priming effects might be accelerated for sites where permafrost degradation leads to the formation of dry thermokarst. C1 [Fan, Zhaosheng; Jastrow, Julie D.; Liang, Chao; Matamala, Roser; Miller, Raymond Michael] Argonne Natl Lab, Biosci Div, Argonne, IL 60439 USA. RP Fan, ZS (reprint author), Argonne Natl Lab, Biosci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM zfan@anl.gov FU U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research, Climate and Environmental Science Division [DE-AC02-06CH11357] FX This work was supported by the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research, Climate and Environmental Science Division under contract DE-AC02-06CH11357. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 64 TC 2 Z9 2 U1 4 U2 56 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD OCT 30 PY 2013 VL 8 IS 10 AR e77880 DI 10.1371/journal.pone.0077880 PG 12 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 243RL UT WOS:000326334500072 PM 24205010 ER PT J AU Bristowe, NC Stengel, M Littlewood, PB Artacho, E Pruneda, JM AF Bristowe, N. C. Stengel, Massimiliano Littlewood, P. B. Artacho, Emilio Pruneda, J. M. TI One-dimensional half-metallic interfaces of two-dimensional honeycomb insulators SO PHYSICAL REVIEW B LA English DT Article ID LOCALIZED WANNIER FUNCTIONS; BORON-NITRIDE; GRAPHENE; ELECTRONICS AB We study zigzag interfaces between insulating compounds that are isostructural to graphene, specifically II-VI, III-V, and IV-IV two-dimensional honeycomb insulators. We show that these one-dimensional interfaces are polar, with a net density of excess charge that can be simply determined by using the ideal (integer) formal valence charges, regardless of the predominant covalent character of the bonding in these materials. We justify this finding on fundamental physical grounds by analyzing the topology of the formal polarization lattice in the parent bulk materials. First-principles calculations elucidate an electronic compensation mechanism not dissimilar to oxide interfaces, which is triggered by a Zener-like charge transfer between interfaces of opposite polarity. In particular, we predict the emergence of one-dimensional electron and hole gases, which in some cases are ferromagnetic half metallic. C1 [Bristowe, N. C.; Littlewood, P. B.; Artacho, Emilio] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bristowe, N. C.] Univ Liege, B-4000 Sart Tilman Par Liege, Belgium. [Stengel, Massimiliano] Inst Catalana Recerca & Estudis Avancats, Barcelona 08010, Spain. [Stengel, Massimiliano] CSIC, Inst Ciencia Mat Barcelona, Bellaterra 08193, Spain. [Littlewood, P. B.] Argonne Natl Lab, Argonne, IL 60439 USA. [Artacho, Emilio] CIC Nanogune & DIPC, San Sebastian 20018, Spain. [Artacho, Emilio] Basque Fdn Sci Ikerbasque, Bilbao 48011, Spain. [Pruneda, J. M.] ICN2 Inst Catala Nanociencia & Nanotecnol, Bellaterra, Barcelona, Spain. [Pruneda, J. M.] CSIC, Bellaterra 08193, Barcelona, Spain. RP Bristowe, NC (reprint author), Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. RI Pruneda, Miguel/A-4077-2008; Stengel, Massimiliano/E-2934-2010; Bristowe, Nicholas/B-2230-2013; Artacho, Emilio/G-2616-2015; DONOSTIA INTERNATIONAL PHYSICS CTR., DIPC/C-3171-2014; nanoGUNE, CIC/A-2623-2015 OI Pruneda, Miguel/0000-0002-3621-6095; Stengel, Massimiliano/0000-0003-4175-3888; Bristowe, Nicholas/0000-0003-1286-8440; Artacho, Emilio/0000-0001-9357-1547; FU EPSRC; MCINN [FIS2009-12721-C0-401, CSD2007-00041]; Spanish Supercomputer Network; HPC Europa; DOE [FWP 70069] FX We acknowledge I. Souza for valuable discussions, the support of EPSRC, MCINN (Grants No. FIS2009-12721-C0-401 and No. CSD2007-00041), and computing resources of CamGRID and Darwin at Cambridge, the Spanish Supercomputer Network, and HPC Europa. P.B.L. acknowledges DOE support under Grant No. FWP 70069. NR 40 TC 9 Z9 9 U1 2 U2 44 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 30 PY 2013 VL 88 IS 16 AR UNSP 161411 DI 10.1103/PhysRevB.88.161411 PG 5 WC Physics, Condensed Matter SC Physics GA 242VW UT WOS:000326273500001 ER PT J AU Liu, XH Wang, Y Burton, JD Tsymbal, EY AF Liu, Xiaohui Wang, Yong Burton, J. D. Tsymbal, Evgeny Y. TI Polarization-controlled Ohmic to Schottky transition at a metal/ferroelectric interface SO PHYSICAL REVIEW B LA English DT Article ID MULTIFERROIC TUNNEL-JUNCTIONS; FERROELECTRIC CONTROL; SPIN POLARIZATION; OXIDE INTERFACES; BIFEO3; HETEROSTRUCTURES; FILMS; PHYSICS; DIODE AB Ferroelectric polar displacements have recently been observed in conducting electron-doped BaTiO3 (n-BTO). The coexistence of a ferroelectric phase and conductivity opens the door to new functionalities that may provide a unique route for novel device applications. Using first-principles methods and electrostatic modeling, we explore the effect that the switchable polarization of n-BTO has on the electronic properties of the SrRuO3/n-BTO (001) interface. Ferroelectric polarization controls the accumulation or depletion of electron charge at the interface, and the associated bending of the n-BTO conduction band determines the transport regime across the interface. The interface exhibits a Schottky tunnel barrier for one polarization orientation, whereas an Ohmic contact is present for the opposite polarization orientation, leading to a large change in interface resistance associated with polarization reversal. Our calculations reveal a five orders of magnitude change in the interface resistance because of polarization switching. C1 [Liu, Xiaohui; Burton, J. D.; Tsymbal, Evgeny Y.] Univ Nebraska, Dept Phys & Astron, Lincoln, NE 68588 USA. [Liu, Xiaohui; Burton, J. D.; Tsymbal, Evgeny Y.] Univ Nebraska, Nebraska Ctr Mat & Nanosci, Lincoln, NE 68588 USA. [Wang, Yong] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. RP Liu, XH (reprint author), Univ Nebraska, Dept Phys & Astron, Lincoln, NE 68588 USA. EM jdburton1@gmail.com; tsymbal@unl.edu RI Tsymbal, Evgeny/G-3493-2013; Burton, John/B-5875-2008 OI Burton, John/0000-0001-5535-2407 FU Nanoelectronics Research Initiative (NRI) through the Center for NanoFerroic Devices (CNFD); US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering (DOE) [DE-SC0004876] FX This research was supported by the Nanoelectronics Research Initiative (NRI) through the Center for NanoFerroic Devices (CNFD) and US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering (DOE Grant No. DE-SC0004876). Computations were performed at the University of Nebraska Holland Computing Center. NR 43 TC 25 Z9 25 U1 8 U2 112 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 30 PY 2013 VL 88 IS 16 AR 165139 DI 10.1103/PhysRevB.88.165139 PG 6 WC Physics, Condensed Matter SC Physics GA 242VW UT WOS:000326273500004 ER PT J AU Shin, CS Avalos, CE Butler, MC Wang, HJ Seltzer, SJ Liu, RB Pines, A Bajaj, VS AF Shin, Chang S. Avalos, Claudia E. Butler, Mark C. Wang, Hai-Jing Seltzer, Scott J. Liu, Ren-Bao Pines, Alexander Bajaj, Vikram S. TI Suppression of electron spin decoherence of the diamond NV center by a transverse magnetic field SO PHYSICAL REVIEW B LA English DT Article ID NITROGEN-VACANCY SPIN; COHERENT DYNAMICS; BATH; RESONANCE; MAGNETOMETRY; QUBITS; TIME AB We demonstrate that the spin decoherence of nitrogen vacancy (NV) centers in diamond can be suppressed by a transverse magnetic field if the electron spin bath is the primary decoherence source. The NV spin coherence, created in "a decoherence-free subspace," is protected by the transverse component of the zero-field splitting, increasing the spin-coherence time about twofold. The decoherence due to the electron spin bath is also suppressed at magnetic fields stronger than similar to 25 G when applied parallel to the NV symmetry axis. Our method can be used to extend the spin-coherence time of similar spin systems for applications in quantum computing, field sensing, and other metrologies. C1 [Shin, Chang S.; Avalos, Claudia E.; Butler, Mark C.; Wang, Hai-Jing; Seltzer, Scott J.; Pines, Alexander; Bajaj, Vikram S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Shin, Chang S.; Avalos, Claudia E.; Butler, Mark C.; Wang, Hai-Jing; Seltzer, Scott J.; Pines, Alexander; Bajaj, Vikram S.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Shin, Chang S.; Avalos, Claudia E.; Butler, Mark C.; Wang, Hai-Jing; Seltzer, Scott J.; Pines, Alexander; Bajaj, Vikram S.] Univ Calif Berkeley, Calif Inst Quantitat Biosci, Berkeley, CA 94720 USA. [Liu, Ren-Bao] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Liu, Ren-Bao] Chinese Univ Hong Kong, Ctr Quantum Coherence, Shatin, Hong Kong, Peoples R China. RP Shin, CS (reprint author), Halliburton Energy Serv Inc, 3000 N Sam Houston Pkwy E, Houston, TX 77032 USA. EM vikbajaj@gmail.com RI Liu, Ren-Bao/B-3729-2011; OI Liu, Ren-Bao/0000-0002-0620-2370; Butler, Mark/0000-0002-1273-5771 FU Office of Science Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U.S. Department of Energy [DE-AC02-05CH11231]; National Science Foundation [CHE-0957655]; Hong Kong RGC-NSFC [N_CUHK403/11] FX The authors thank Ran Fischer and Dmitry Budker for useful discussions. This work was supported by the Director, Office of Science Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. M.B. acknowledges financial support from the National Science Foundation under Award No. CHE-0957655. R.L. acknowledges financial support from Hong Kong RGC-NSFC Project N_CUHK403/11. NR 39 TC 6 Z9 6 U1 0 U2 29 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 30 PY 2013 VL 88 IS 16 AR 161412 DI 10.1103/PhysRevB.88.161412 PG 5 WC Physics, Condensed Matter SC Physics GA 242VW UT WOS:000326273500002 ER PT J AU Hu, XF Wu, J Niu, DX Chen, L Morton, SA Scholl, A Huang, ZC Zhai, Y Zhang, W Will, I Xu, YB Zhang, R van der Laan, G AF Hu, X. F. Wu, J. Niu, D. X. Chen, L. Morton, S. A. Scholl, A. Huang, Z. C. Zhai, Y. Zhang, W. Will, I. Xu, Y. B. Zhang, R. van der Laan, G. TI Discontinuous properties of current-induced magnetic domain wall depinning SO SCIENTIFIC REPORTS LA English DT Article DE APPLIED PHYSICS; MAGNETIC DEVICES; SPINTRONICS; FERROMAGNETISM ID MOTION; NANOWIRES; DYNAMICS; STRIPS AB The current-induced motion of magnetic domain walls (DWs) confined to nanostructures is of great interest for fundamental studies as well as for technological applications in spintronic devices. Here, we present magnetic images showing the depinning properties of pulse-current-driven domain walls in well-shaped Permalloy nanowires obtained using photoemission electron microscopy combined with x-ray magnetic circular dichroism. In the vicinity of the threshold current density (Jth = 4.2 x 10(11) A.m(-2)) for the DW motion, discontinuous DW depinning and motion have been observed as a sequence of "Barkhausen jumps". A one-dimensional analytical model with a piecewise parabolic pinning potential has been introduced to reproduce the DW hopping between two nearest neighbour sites, which reveals the dynamical nature of the current-driven DW motion in the depinning regime. C1 [Hu, X. F.; Niu, D. X.; Zhang, W.; Will, I.; Xu, Y. B.] Univ York, Dept Elect, Spintron & Nanodevice Lab, York YO10 5DD, N Yorkshire, England. [Hu, X. F.; Wu, J.; Niu, D. X.; Xu, Y. B.; Zhang, R.] Nanjing Univ, Sch Elect Sci & Engn, Nanjing York Int Ctr Spintron, Nanjing 210093, Jiangsu, Peoples R China. [Wu, J.] Univ York, Dept Phys, York YO10 5DD, N Yorkshire, England. [Chen, L.] Univ Leeds, Dept Elect, Leeds LS2 9JT, W Yorkshire, England. [Morton, S. A.; Scholl, A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Huang, Z. C.; Zhai, Y.] Southeast Univ, Dept Phys, Nanjing 211189, Jiangsu, Peoples R China. [van der Laan, G.] Magnet Spect Grp, Diamond Light Source, Didcot OX11 0DE, Oxon, England. RP Xu, YB (reprint author), Univ York, Dept Elect, Spintron & Nanodevice Lab, York YO10 5DD, N Yorkshire, England. EM yongbing.xu@york.ac.uk RI Scholl, Andreas/K-4876-2012; van der Laan, Gerrit/Q-1662-2015; Zhai, Ya/J-6991-2012; OI van der Laan, Gerrit/0000-0001-6852-2495; Zhai, Ya/0000-0002-9006-9575; Huang, Zhaocong/0000-0002-0190-2810 FU State Key Programme for Basic Research of China [2014CB921101]; NSFC [61274102]; PAPD project; UK EPSRC; STFC; Office of Science, Office of Basic Energy Sciences, of the US Department of Energy [DE-AC02-05CH11231] FX This work is supported by the State Key Programme for Basic Research of China (Grants No. 2014CB921101), NSFC (Grants No. 61274102) and PAPD project, UK EPSRC and STFC. The Advanced Light Source at Lawrence Berkeley National Laboratory is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the US Department of Energy under Contract No. DE-AC02-05CH11231. XH would like to thank the York NanoCenter for samples fabrication support. NR 51 TC 3 Z9 3 U1 4 U2 53 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD OCT 30 PY 2013 VL 3 AR 3080 DI 10.1038/srep03080 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 243QR UT WOS:000326332500001 PM 24170087 ER PT J AU Nicholson, DM Ojha, M Egami, T AF Nicholson, D. M. Ojha, Madhusudan Egami, T. TI First-principles local stress in crystalline and amorphous metals SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article ID DENSITY; ENERGY AB Atomic size is perhaps the most commonly used concept to describe material properties. Advances in the understanding of materials are hindered by the available choices of simplifying concepts that can be used. However, the precise definition of atomic size is not easy, and often controversial. Atomic level stress provides a new interpretive tool that draws on the rich formalism of solid mechanics for use with density functional calculations to advance a deeper understanding of the properties of materials. We discuss atomic level stresses in liquids and glasses and make comparisons with ordered and disordered crystals. Somewhat surprisingly, even ordered compounds that are under no macroscopic stress and whose individual atoms are completely relaxed, i.e., no force acting on them, can have substantial atomic level stresses. On top of concepts such as the ionicity or covalency, the atomic level stresses add to the arsenal of analysis tools that are available to interpret the results of density functional calculations. C1 [Nicholson, D. M.; Ojha, Madhusudan; Egami, T.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Ojha, Madhusudan; Egami, T.] Univ Tennessee, Knoxville, TN 37996 USA. RP Nicholson, DM (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. EM nicholsondm@ornl.gov FU US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division; Office of Science of the US Department of Energy [DE-AC02-05CH11231] FX Research at ORNL was supported by the US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the US Department of Energy under Contract No. DE-AC02-05CH11231. NR 24 TC 3 Z9 3 U1 3 U2 29 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD OCT 30 PY 2013 VL 25 IS 43 AR 435505 DI 10.1088/0953-8984/25/43/435505 PG 11 WC Physics, Condensed Matter SC Physics GA 237UR UT WOS:000325896900012 PM 24107600 ER PT J AU Tomic, S Pinteric, M Ivek, T Sedlmeier, K Beyer, R Wu, D Schlueter, JA Schweitzer, D Dressel, M AF Tomic, S. Pinteric, M. Ivek, T. Sedlmeier, K. Beyer, R. Wu, D. Schlueter, J. A. Schweitzer, D. Dressel, M. TI Magnetic ordering and charge dynamics in kappa-(BEDT-TTF)(2)Cu [N(CN)(2)]Cl SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article ID ORGANIC CONDUCTORS; BEDT-TTF; DENSITY WAVES; BIS(ETHYLENEDITHIO)TETRATHIAFULVALENE; PHASE; RAMAN; VIBRATIONS; ANISOTROPY; MODEL; NMR AB The Mott insulator kappa-(BEDT-TTF)(2)Cu[N(CN)(2)]Cl consists of molecular dimers arranged on an anisotropic triangular lattice. At low temperatures a pronounced dielectric anomaly is observed, and eventually a canted antiferromagnetic ground state forms. Optical spectroscopy clearly rules out charge imbalance and the existence of quantum electric dipoles with a dipolar-spin coupling. Here we suggest a novel form of spin-charge coupling where the prominent in-plane dielectric response in kappa-(BEDT-TTF)(2)Cu[N(CN)(2)]Cl is explained by short-range discommensurations of the antiferromagnetic phase in the temperature range 30 K < T < 50 K, and by relaxation of charged domain walls in the ferromagnetic structure at lower temperatures. C1 [Tomic, S.; Pinteric, M.; Ivek, T.] Inst Fiziku, HR-10001 Zagreb, Croatia. [Pinteric, M.] Univ Maribor, Fac Civil Engn, SLO-2000 Maribor, Slovenia. [Ivek, T.; Sedlmeier, K.; Beyer, R.; Wu, D.; Schweitzer, D.; Dressel, M.] Univ Stuttgart, Inst Phys, D-70550 Stuttgart, Germany. [Schlueter, J. A.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Tomic, S (reprint author), Inst Fiziku, POB 304, HR-10001 Zagreb, Croatia. EM stomic@ifs.hr RI Tomic, Silvia/D-5466-2011; Ivek, Tomislav/D-5298-2011; Dressel, Martin/D-3244-2012; Pinteric, Marko/D-5739-2011 FU Deutsche Forschungsgemeinschaft (DFG); Deutscher Akademische Auslandsdienst (DAAD); Croatian Ministry of Science, Education and Sports [035-0000000-2836] FX We thank C Hotta, K Kanoda, S Mazumdar, J-P. Pouget, E Rose, M Tanatar, E Tutis and T Yamamoto for helpful discussions. The project was supported by the Deutsche Forschungsgemeinschaft (DFG), the Deutscher Akademische Auslandsdienst (DAAD) and the Croatian Ministry of Science, Education and Sports under grant 035-0000000-2836. NR 50 TC 9 Z9 9 U1 1 U2 33 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD OCT 30 PY 2013 VL 25 IS 43 AR 436004 DI 10.1088/0953-8984/25/43/436004 PG 7 WC Physics, Condensed Matter SC Physics GA 237UR UT WOS:000325896900023 PM 24107640 ER PT J AU Aad, G Abajyan, T Abbott, B Abdallah, J Khalek, SA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Addy, TN Adelman, J Adomeit, S Adye, T Aefsky, S Agatonovic-Jovin, T Aguilar-Saavedra, JA Agustoni, M Ahlen, SP Ahmad, A Ahsan, M Aielli, G Akesson, TPA Akimoto, G Akimov, AV Alam, MA Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alessandria, F Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Aliev, M Alimonti, G Alio, L Alison, J Allbrooke, BMM Allison, LJ Allport, PP Allwood-Spiers, SE Almond, J Aloisio, A Alon, R Alonso, A Alonso, F Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Coutinho, YA Amelung, C Ammosov, VV Dos Santos, SPA Amorim, A Amoroso, S Amram, N Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Anduaga, XS Angelidakis, S Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonaki, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Apolle, R Arabidze, G Aracena, I Arai, Y Arce, ATH Arfaoui, S Arguin, JF Argyropoulos, S Arik, E Arik, M Armbruster, AJ Arnaez, O Arnal, V Arslan, O Artamonov, A Artoni, G Arutinov, D Asai, S Asbah, N Ask, S Asman, B Asquith, L Assamagan, K Astalos, R Astbury, A Atkinson, M Atlay, NB Auerbach, B Auge, E Augsten, K Aurousseau, M Avolio, G Axen, D Azuelos, G Azuma, Y Baak, MA Bacci, C Bach, AM Bachacou, H Bachas, K Backes, M Backhaus, M Mayes, JB Badescu, E Bagiacchi, P Bagnaia, P Bai, Y Bailey, DC Bain, T Baines, JT Baker, OK Baker, S Balek, P Balli, F Banas, E Banerjee, S Banfi, D Bangert, A Bansal, V Bansil, HS Barak, L Baranov, SP Barber, T Barberio, EL Barberis, D Barbero, M Bardin, DY Barillari, T Barisonzi, M Barklow, T Barlow, N Barnett, BM Barnett, RM Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartsch, V Basye, A Bates, RL Batkova, L Batley, JR Battistin, M Bauer, F Bawa, HS Beale, S Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, S Beckingham, M Becks, KH Beddall, AJ Beddall, A Bedikian, S Bednyakov, VA Bee, CP Beemster, LJ Beermann, TA Begel, M Belanger-Champagne, C Bell, PJ Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belloni, A Beloborodova, OL Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Benslama, K Bentvelsen, S Berge, D Kuutmann, EB Berger, N Berghaus, F Berglund, E Beringer, J Bernard, C Bernat, P Bernhard, R Bernius, C Bernlochner, FU Berry, T Bertella, C Bertolucci, F Besana, MI Besjes, GJ Bessidskaia, O Besson, N Bethke, S Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Bieniek, SP Bierwagen, K Biesiada, J Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Bittner, B Black, CW Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blazek, T Bloch, I Blocker, C Blocki, J Blum, W Blumenschein, U Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Boddy, CR Boehler, M Boek, J Boek, TT Boelaert, N Bogaerts, JA Bogdanchikov, AG Bogouch, A Bohm, C Bohm, J Boisvert, V Bold, T Boldea, V Bolnet, NM Bomben, M Bona, M Boonekamp, M Bordoni, S Borer, C Borisov, A Borissov, G Borri, M Borroni, S Bortfeldt, J Bortolotto, V Bos, K Boscherini, D Bosman, M Boterenbrood, H Bouchami, J Boudreau, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boutouil, S Boveia, A Boyd, J Boyko, IR Bozovic-Jelisavcic, I Bracinik, J Branchini, P Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Brazzale, SF Brelier, B Bremer, J Brendlinger, K Brenner, R Bressler, S Bristow, TM Britton, D Brochu, FM Brock, I Brock, R Broggi, F Bromberg, C Bronner, J Brooijmans, G Brooks, T Brooks, WK Brost, E Brown, G Brown, J de Renstrom, PAB Bruncko, D Bruneliere, R Brunet, S Bruni, A Bruni, G Bruschi, M Bryngemark, L Buanes, T Buat, Q Bucci, F Buchanan, J Buchholz, P Buckingham, RM Buckley, AG Buda, SI Budagov, IA Budick, B Buehrer, F Bugge, L Bulekov, O Bundock, AC Bunse, M Buran, T Burckhart, H Burdin, S Burgess, T Burke, S Busato, E Uscher, VB Bussey, P Buszello, CP Butler, B Butler, JM Buttar, CM Butterworth, JM Buttinger, W Byszewski, M Urbaan, SC Caforio, D Cakir, O Calafiura, P Calderini, G Calfayan, P Calkins, R Caloba, LP Caloi, R Calvet, D Calvet, S Toro, RC Camarri, P Cameron, D Caminada, LM Armadans, RC Campana, S Campanelli, M Canale, V Canelli, F Canepa, A Cantero, J Cantrill, R Cao, T Garrido, MDMC Caprini, I Caprini, M Capriotti, D Capua, M Caputo, R Cardarelli, R Carli, T Carlino, G Carminati, L Caron, S Carquin, E Carrillo-Montoya, GD Carter, AA Carter, JR Carvalho, J Casadei, D Casado, MP Caso, C Castaneda-Miranda, E Castelli, A Gimenez, VC Castro, NF Cataldi, G Catastini, P Catinaccio, A Catmore, JR Cattai, A Cattani, G Caughron, S Cavaliere, V Cavalli, D Cavalli-Sforza, M Cavasinni, V Ceradini, F Cerio, B Cerqueira, AS Cerri, A Cerrito, L Cerutti, F Cervelli, A Cetin, SA Chafaq, A Chakraborty, D Chalupkova, I Chan, K Chang, P Chapleau, B Chapman, JD Chapman, JW Charlton, DG Chavda, V Barajas, CAC Cheatham, S Chekanov, S Chekulaev, SV Chelkov, GA Chelstowska, MA Chen, C Chen, H Chen, S Chen, X Chen, Y Cheng, Y Cheplakov, A El Moursli, RC Chernyatin, V Cheu, E Chevalier, L Chiarella, V Chiefari, G Childers, JT Chilingarov, A Chiodini, G Chisholm, AS Chislett, RT Chitan, A Chizhov, MV Choudalakis, G Chouridou, S Chow, BKB Christidi, IA Christov, A Chromek-Burckhart, D Chu, ML Chudoba, J Ciapetti, G Ciftci, AK Ciftci, R Cinca, D Cindro, V Ciocio, A Cirilli, M Cirkovic, P Citron, ZH Citterio, M Ciubancan, M Clark, A Clark, PJ Clarke, RN Clemens, JC Clement, B Clement, C Coadou, Y Cobal, M Coccaro, A Cochran, J Coelli, S Coffey, L Cogan, JG Coggeshall, J Colas, J Cole, B Cole, S Colijn, AP Collins-Tooth, C Collot, J Colombo, T Colon, G Compostella, G Muino, PC Coniavitis, E Conidi, MC Consonni, SM Consorti, V Constantinescu, S Conta, C Conti, G Conventi, F Cooke, M Cooper, BD Cooper-Sarkar, AM Cooper-Smith, NJ Copic, K Cornelissen, T Corradi, M Corriveau, F Corso-Radu, A Cortes-Gonzalez, A Cortiana, G Costa, G Costa, MJ Costanzo, D Cote, D Cottin, G Courneyea, L Cowan, G Cox, BE Cranmer, K Crepe-Renaudin, S Crescioli, F Cristinziani, M Crosetti, G Cuciuc, CM Almenar, CC Donszelmann, TC Cummings, J Curatolo, M Cuthbert, C Czirr, H Czodrowski, P Czyczula, Z D'Auria, S D'Onofrio, M D'Orazio, A De Sousa, MJDS Da Via, C Dabrowski, W Dafinca, A Dai, T Dallaire, F Dallapiccola, C Dam, M Damiani, DS Daniells, AC Dao, V Darbo, G Darlea, GL Darmora, S Dassoulas, JA Davey, W David, C Davidek, T Davies, E Davies, M Davignon, O Davison, AR Davygora, Y Dawe, E Dawson, I Daya-Ishmukhametova, RK De, K de Asmundis, R De Castro, S De Cecco, S de Graat, J De Groot, N de 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Wotschack, J. Woudstra, M. J. Wozniak, K. W. Wraight, K. Wright, M. Wrona, B. Wu, S. L. Wu, X. Wu, Y. Wulf, E. Wynne, B. M. Xella, S. Xiao, M. Xu, C. Xu, D. Xu, L. Yabsley, B. Yacoob, S. Yamada, M. Yamaguchi, H. Yamaguchi, Y. Yamamoto, A. Yamamoto, K. Yamamoto, S. Yamamura, T. Yamanaka, T. Yamauchi, K. Yamazaki, Y. Yan, Z. Yang, H. Yang, H. Yang, U. K. Yang, Y. Yang, Z. Yanush, S. Yao, L. Yasu, Y. Yatsenko, E. Wong, K. H. Yau Ye, J. Ye, S. Yen, A. L. Yildirim, E. Yilmaz, M. Yoosoofmiya, R. Yorita, K. Yoshida, R. Yoshihara, K. Young, C. Young, C. J. S. Youssef, S. Yu, D. R. Yu, J. Yu, J. Yuan, L. Yurkewicz, A. Zabinski, B. Zaidan, R. Zaitsev, A. M. Zambito, S. Zanello, L. Zanzi, D. Zaytsev, A. Zeitnitz, C. Zeman, M. Zemla, A. Zenin, O. Zenis, T. Zerwas, D. della Porta, G. Zevi Zhang, D. Zhang, H. Zhang, J. Zhang, L. Zhang, X. Zhang, Z. Zhao, Z. Zhemchugov, A. Zhong, J. Zhou, B. Zhou, N. Zhu, C. G. Zhu, H. Zhu, J. Zhu, Y. Zhuang, X. Zibell, A. Zieminska, D. Zimin, N. I. Zimmermann, C. Zimmermann, R. Zimmermann, S. Zimmermann, S. Zinonos, Z. Ziolkowski, M. Zitoun, R. Zivkovic, L. Zobernig, G. Zoccoli, A. Nedden, M. zur Zurzolo, G. Zutshi, V. Zwalinski, L. CA ATLAS Collaboration TI Search for direct third-generation squark pair production in final states with missing transverse momentum and two b-jets in root s=8 TeV pp collisions with the ATLAS detector SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering; Supersymmetry ID DYNAMICAL SYMMETRY-BREAKING; SUPERGAUGE TRANSFORMATIONS; SUPERSYMMETRY; MODEL; PARTICLE; CURRENTS; LEPTONS; MASSES; QUARKS; PIONS AB The results of a search for pair production of supersymmetric partners of the Standard Model third-generation quarks are reported. This search uses 20.1 fb(-1) of pp collisions at root s = 8 TeV collected by the ATLAS experiment at the Large Hadron Collider. The lightest bottom and top squarks ((b) over tilde (1) and (t) over tilde (1) respectively) are searched for in a final state with large missing transverse momentum and two jets identified as originating from b-quarks. No excess of events above the expected level of Standard Model background is found. The results are used to set upper limits on the visible cross section for processes beyond the Standard Model. Exclusion limits at the 95% confidence level on the masses of the third-generation squarks are derived in phenomenological supersymmetric R-parity-conserving models in which either the bottom or the top squark is the lightest squark. The (b) over tilde (1) is assumed to decay via (b) over tilde (1) -> b (chi) over tilde (0)(1) and the (t) over tilde (1) via (t) over tilde (1) b (chi) over tilde (+/-)(1), with undetectable products of the subsequent decay of the (chi) over tilde (+/-)(1) due to the small mass splitting between the (chi) over tilde (+/-)(1) and the (chi) over tilde (0)(1) C1 [Jackson, P.; Soni, N.] Univ Adelaide, Sch Chem & Phys, Adelaide, SA, Australia. [Edson, W.; Ernst, J.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY USA. [Chan, K.; Gingrich, D. M.; Moore, R. W.; Pinfold, J. L.; Saddique, A.; Sbrizzi, A.; Subramania, H. S.; Vaque, F. Vives] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakir, O.; Ciftci, A. K.; Ciftci, R.; Yildiz, H. Duran; Kuday, S.] Ankara Univ, Dept Phys, TR-06100 Ankara, Turkey. [Yilmaz, M.] Gazi Univ, Dept Phys, Ankara, Turkey. [Sultansoy, S.] TOBB Univ Econ & Technol, Div Phys, Ankara, Turkey. [Cakir, I. Turk] Turkish Atom Energy Commiss, Ankara, Turkey. 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[Alison, J.; Anderson, K. J.; Boveia, A.; Canelli, F.; Cheng, Y.; Choudalakis, G.; Fiascaris, M.; Gardner, R. W.; Plante, I. Jen-La; Kapliy, A.; Li, H. L.; Meehan, S.; Melachrinos, C.; Merritt, F. S.; Meyer, C.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Shochet, M. J.; Tompkins, L.; Tuggle, J. M.; Vukotic, I.; Webster, J. S.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Cottin, G.; Diaz, M. A.] Pontificia Univ Catolica Chile, Fac Fis, Santiago 22, Chile. [Brooks, W. K.; Carquin, E.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; White, R.] Univ Tecn Feder Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Huang, Y.; Jin, S.; Lu, F.; Ouyang, Q.; Shan, L. Y.; Wang, J.; Xu, D.; Yao, L.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Han, L.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, K.; Liu, M.; Liu, Y.; Peng, H.; Xu, C.; Xu, L.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Yang, H.] Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200030, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Karpov, S. N.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Clermont Univ, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Karpov, S. N.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Karpov, S. N.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] CNRS, IN2P3, Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Chen, Y.; Cole, B.; Dodd, J.; Guo, J.; Hu, D.; Hughes, E. W.; Kohriki, T.; Metcalfe, J.; Nikiforou, N.; Parsons, J. A.; Penson, A.; Perepelitsa, D. V.; Reale, V. Perez; Scherzer, M. I.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Williams, E.; Willis, W.; Wulf, E.; Zivkovic, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Boelaert, N.; Dam, M.; Galster, G.; Gregersen, K.; Hansen, J. R.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Heisterkamp, S.; Jakobsen, S.; Joergensen, M. D.; Kadlecik, P.; Klinkby, E. B.; Loevschall-Jensen, A. E.; Mackeprang, R.; Mehlhase, S.; Monk, J.; Petersen, T. C.; Pingel, A.; Simonyan, M.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Policicchio, A.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Grp Coll Cosenza, Arcavacata Di Rende, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Policicchio, A.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartmento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; Blocki, J.; de Renstrom, P. A. Bruckman; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.; Zemla, A.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Cao, T.; Yagci, K. Dindar; Firan, A.; Hoffman, J.; Joffe, D.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Rios, R. R.; Sekula, S. J.; Stroynowski, R.; Wang, H.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Ahsan, M.; Izen, J. M.; Lou, X.; Namasivayam, H.; Reeves, K.; Wong, W. C.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Dassoulas, J. A.; Dietrich, J.; Ferrara, V.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Goebel, M.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Hiller, K. H.; Huettmann, A.; Belenguer, M. Jimenez; Johnert, S.; Katzy, J.; Kono, T.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Cavalcanti, T. Perez; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.; Zhu, H.] DESY, Hamburg, Germany. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Dassoulas, J. A.; Dietrich, J.; Ferrara, V.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Goebel, M.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Hiller, K. H.; Huettmann, A.; Belenguer, M. Jimenez; Johnert, S.; Katzy, J.; Kono, T.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Cavalcanti, T. Perez; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.; Zhu, H.] DESY, Zeuthen, Germany. [Buckley, A. G.; Bunse, M.; Esch, H.; Gossling, C.; Harrington, R. D.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Reisinger, I.; Wittig, T.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Czodrowski, P.; Friedrich, F.; Grohs, J. P.; Kobel, M.; Leonhardt, K.; Mader, W. F.; Morgenstern, M.; Prudent, X.; Rudolph, C.; Schnoor, U.; Seifert, F.; Steinbach, P.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B.; Finelli, K. D.; Ko, B. R.; Kotwal, A.; Kruse, M. K.; Li, S.; Liu, M.; Oh, S. H.; Pollard, C. S.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Debenedetti, C.; Edwards, N. C.; Walls, F. M. Garay; Korn, A.; Martin, V. J.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Schaelicke, A.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, Sch Phys & Astron, SUPA, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.; Volpi, G.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Aad, G.; Amoroso, S.; Barber, T.; Bernhard, R.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Christov, A.; Consorti, V.; Di Simone, A.; Fehling-Kaschek, M.; Flechl, M.; Giuliani, C.; Hartert, J.; Herten, G.; Jakobs, K.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Lohwasser, K.; Ludwig, I.; Ludwig, J.; Madar, R.; Mahboubi, K.; Mohr, W.; Parzefall, U.; Rammensee, M.; Rave, T. C.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Siegert, F.; Stoerig, K.; Sundermann, J. E.; Temming, K. K.; Thoma, S.; Tsiskaridze, V.; Ungaro, F. C.; Venturi, M.; Vivarelli, I.; von Radziewski, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Winkelmann, S.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, Freiburg, Germany. [Alexandre, G.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Bucci, F.; Toro, R. Camacho; Clark, A.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; dit Latour, B. Martin; Mermod, P.; Herrera, C. Mora; Muenstermann, D.; Nektarijevic, S.; Nikolics, K.; Pasztor, G.; Picazio, A.; Pohl, M.; Rosbach, K.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Beccherle, R.; Caso, C.; Darbo, G.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Genoa, Italy. [Barberis, D.; Caso, C.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Khubua, J.; Mchedlidze, G.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Bussey, P.; Buttar, C. M.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Quilty, D.; Ravenscroft, T.; Robson, A.; Saxon, D. H.; Snow, J.; Denis, R. D. St.; Steele, G.; Thompson, A. S.; Wraight, K.; Wright, M.] Univ Glasgow, Sch Phys & Astron, SUPA, Glasgow, Lanark, Scotland. [Bierwagen, K.; Blumenschein, U.; Brandt, O.; Evangelakou, D.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Hensel, C.; Kawamura, G.; Keil, M.; Knue, A.; Kohn, F.; Krieger, N.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Meyer, J.; Morel, J.; Nackenhorst, O.; Pashapour, S.; Peters, R. F. Y.; Quadt, A.; Roe, A.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Schroeder, T. Vazquez; Weingarten, J.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Brown, J.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] Univ Grenoble 1, Lab Phys Subatom & Cosmol, Grenoble, France. [Albrand, S.; Brown, J.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] CNRS, IN2P3, Grenoble, France. [Albrand, S.; Brown, J.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] Inst Natl Polytechn Grenoble, Grenoble, France. [Addy, T. N.; Harvey, A.; McFarlane, K. W.; Shin, T.; Vassilakopoulos, V. I.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Belloni, A.; Butler, B.; Catastini, P.; Conti, G.; Franklin, M.; Huth, J.; Jeanty, L.; Mateos, D. Lopez; Mercurio, K. M.; Mills, C.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Yen, A. L.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Anders, G.; Andrei, V.; Davygora, Y.; Dietzsch, T. A.; Dunford, M.; Hofmann, J. I.; Khomich, A.; Kluge, E. -E.; Laier, H.; Lang, V. S.; Lendermann, V.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, D-69115 Heidelberg, Germany. [Anders, C. F.; Kasieczka, G.; Narayan, R.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, D-69115 Heidelberg, Germany. [Kugel, A.; Schroer, N.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Evans, H.; Gagnon, P.; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Price, D.; Whittington, D.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jussel, P.; Kneringer, E.; Lukas, W.; Nagai, K.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Cinca, D.; Gandrajula, R. P.; Halladjian, G.; Limper, M.; Mallik, U.; Mandrysch, R.; Morange, N.; Pylypchenko, Y.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Ruiz-Martinez, A.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Aleksandrov, I. N.; Bardin, D. Y.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Goestkin, M. I.; Grigalashvili, N.; Huseynov, N.; Kazarinov, M. Y.; Kharchenko, D.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rumyantsev, L.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.; Zimin, N. I.] Joint Inst Nucl Res Dubna, Dubna, Russia. [Amako, K.; Arai, Y.; Doi, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kondo, T.; Makida, Y.; Mitsui, S.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Shiyakova, M.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [King, M.; Kishimoto, T.; Kitamura, T.; Kurashige, H.; Matsushita, T.; Ochi, A.; Shimizu, S.; Takeda, H.; Tani, K.; Watanabe, I.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Franz, S.; Ishino, M.; Sasao, N.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Verzini, M. J. Alconada; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Argentina. [Verzini, M. J. Alconada; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Consejo Nacl Invest Cient & Tecn, La Plata, Argentina. [Allison, L. J.; Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Bianco, M.; Cataldi, G.; Chiodini, G.; Gorini, E.; Grancagnolo, F.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Bianco, M.; Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Greenshaw, T.; Gwilliam, C. B.; Hayward, H. S.; Jackson, J. N.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Schnellbach, Y. J.; Sellers, G.; Vossebeld, J. H.; Waller, P.; Wrona, B.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Keresevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Keresevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia. [Bona, M.; Carter, A. A.; Cerrito, L.; Eisenhandler, E.; Ellis, K.; Goddard, J. R.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Rizvi, E.; Salamanna, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Alam, M. A.; Berry, T.; Boisvert, V.; Brooks, T.; Cantrill, R.; Cooper-Smith, N. J.; Cowan, G.; Duguid, L.; Edwards, C. A.; George, S.; Gibson, S. M.; Goncalo, R.; Vazquez, J. G. Panduro; Pastore, Fr.; Rose, M.; Spano, F.; Strong, J. A.; Teixeira-Dias, P.] Univ London Royal Holloway & Bedford New Coll, Dept Phys, Egham TW20 0EX, Surrey, England. [Baker, S.; Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christidi, I. A.; Cooper, B. D.; Davison, A. R.; Dobson, E.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Lambourne, L.; Nash, M.; Nurse, E.; Ochoa, M. I.; Pilkington, A. D.; Prabhu, R.; Sherwood, P.; Simmons, B.; Taylor, C.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Bernius, C.; Dhullipudi, R.; Greenwood, Z. D.; Sawyer, L.; Sircar, A.; Subramaniam, R.; Tamsett, M. C.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Jarlskog, G.; Lytken, E.; Meirose, B.; Mjoernmark, J. U.; Smirnova, O.; Snidero, G.; Wielers, M.] Lund Univ, Fys Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Labarga, L.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Arnaez, O.; Blum, W.; Uscher, V. B.; Caputo, R.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Goeringer, C.; Handel, C.; Heck, T.; Hohlfeld, M.; Hsu, P. J.; Huelsing, T. A.; Ji, W.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Meyer, C.; Moreno, D.; Moritz, S.; Mueller, T.; Neusiedl, A.; Poettgen, R.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Almond, J.; Borri, M.; Brown, G.; Chavda, V.; Cox, B. E.; Da Via, C.; Forti, A.; Howarth, J.; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Marx, M.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Robinson, J. E. M.; Tomlinson, L.; Watts, S.; Woudstra, M. J.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Alio, L.; Barbero, M.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Nagai, Y.; Odier, J.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Alio, L.; Barbero, M.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Nagai, Y.; Odier, J.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Brau, B.; Colon, G.; Dallapiccola, C.; Fletcher, G.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Dufour, M-A.; Klemetti, M.; Mantifel, R.; Robertson, S. H.; Schram, M.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Wang, K.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Diglio, S.; Hamano, K.; Jennens, D.; Kubota, T.; Limosani, A.; Hanninger, G. Nunes; Phan, A.; Shao, Q. T.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Volpi, M.; White, M. J.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Armbruster, A. J.; Chapman, J. W.; Chelstowska, M. A.; Cirilli, M.; Dai, T.; Diehl, E. B.; Dubbert, J.; Feng, H.; Ferretti, C.; Goldfarb, S.; Harper, D.; Levin, D.; Li, X.; Liu, L.; Mc Kee, S. P.; Neal, H. A.; Panikashvili, N.; Qian, J.; Scheirich, D.; Searcy, J.; Thun, R. P.; Walch, S.; Wilson, A.; Wooden, G.; Wu, Y.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Hauser, R.; Hayden, D.; Holzbauer, J. L.; Huston, J.; Koll, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schwienhorst, R.; Stelzer, H. J.; Tollefson, K.; True, P.; Warburton, A.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alessandria, F.; Alimonti, G.; Andreazza, A.; Besana, M. I.; Broggi, F.; Carminati, L.; Cavalli, D.; Citterio, M.; Coelli, S.; Consonni, S. M.; Costa, G.; Fanti, M.; Favareto, A.; Giugni, D.; Koletsou, I.; Lari, T.; Mandelli, L.; Mazzanti, M.; Meloni, F.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Rivoltella, G.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Volpini, G.] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Favareto, A.; Meloni, F.; Perini, L.; Pizio, C.; Ragusa, F.; Rivoltella, G.; Simoniello, R.; Turra, R.] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Satsounkevitch, I.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus. [Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Asbah, N.; Azuelos, G.; Bouchami, J.; Dallaire, F.; Davies, M.; Gauthier, L.; Giunta, M.; Leroy, C.; Martin, J. P.; Rezvani, R.; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Sulin, V. V.; Tikhomirov, V. O.] Acad Sci, PN Lebedev Inst Phys, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] ITEP, Moscow, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Smizanska, M.; Soldatov, E. Yu.; Timoshenko, S.] MEPhI, Moscow, Russia. [Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Snesarev, A. A.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Beale, S.; Becker, S.; Biebel, O.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; de Graat, J.; Duckeck, G.; Ebke, J.; Elmsheuser, J.; Engl, A.; Galea, C.; Heller, C.; Hertenberger, R.; Legger, F.; Lorenz, J.; Mann, A.; Meineck, C.; Nunnemann, T.; Oakes, L. B.; Rauscher, F.; Reznicek, P.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Schieck, J.; Schmitt, C.; Staude, A.; Walker, R.; Will, J. Z.; Wittkowski, J.; Zibell, A.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bittner, B.; Bronner, J.; Capriotti, D.; Compostella, G.; Cortiana, G.; Flowerdew, M. J.; Giovannini, P.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kotov, S.; Kroha, H.; Macchiolo, A.; Manfredini, A.; Menke, S.; Moser, H. G.; Nagel, M.; Nisius, R.; Oberlack, H.; Pahl, C.; Pospelov, G. E.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Stern, S.; Stonjek, S.; Vanadia, M.; von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. 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C.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Dao, V.; De Groot, N.; Filthaut, F.; Klok, P. F.; Koenig, A. C.; Raas, M.; Salvucci, A.; Toms, K.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Oussoren, K. P.; Pani, P.; Ruckstuhl, N.; Ta, D.; Tsiakiris, M.; Valencic, N.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. 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V.; Beloborodova, O. L.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Skovpen, K. Yu.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Budick, B.; Cranmer, K.; Haas, A.; van Huysduynen, L. Hooft; Kaplan, B.; Konoplich, R.; Krasznahorkay, A.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.; Prokofiev, K.] NYU, Dept Phys, New York, NY 10003 USA. [Fisher, M. J.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Strang, M.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Gutierrez, P.; Jana, D. K.; Marzin, A.; Meera-Lebbai, R.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. 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Abdel; Auge, E.; Binet, S.; Bourdarios, C.; De La Taille, C.; De Vivie De Regie, J. B.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Teinturier, M.; Tran, H. L.; Zerwas, D.; Zhang, Z.] CNRS, IN2P3, F-91405 Orsay, France. [Hanagaki, K.; Hirose, M.; Lee, J. S. H.; Nomachi, M.; Okamura, W.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Buran, T.; Cameron, D.; Gjelsten, B. K.; Gramstad, E.; Lund, E.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Read, A. L.; Rohne, O.; Smestad, L.; Smith, K. M.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Apolle, R.; Barr, A. J.; Boddy, C. R.; Buchanan, J.; Buckingham, R. M.; Cooper-Sarkar, A. M.; Dafinca, A.; Davies, E.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; King, R. S. B.; Kogan, L. A.; Larner, A.; Lewis, A.; Livermore, S. S. A.; Mattravers, C.; Nickerson, R. B.; Pachal, K.; Pinder, A.; Robichaud-Veronneau, A.; Ryder, N. C.; Sawyer, C.; Short, D.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Young, C. J. S.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Colombo, T.; Conta, C.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Colombo, T.; Conta, C.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Degenhardt, J.; Fratina, S.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Keener, P. T.; Kroll, J.; Kunkle, J.; Lester, C. 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Amor; Amorim, A.; Anjos, N.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; Da Cunha Sargedas De Sousa, M. J.; Wemans, A. Do Valle; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Jorge, P. M.; Lopes, L.; Miguens, J. Machado; Maio, A.; Maneira, J.; Marques, C. N.; Oliveira, M.; Onofre, A.; Palma, A.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. [Bohm, J.; Chudoba, J.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Myska, M.; Nemecek, S.; Ruzicka, P.; Schovancova, J.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Tic, T.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Gallus, P.; Gunther, J.; Jakubek, J.; Kohout, Z.; Kral, V.; Pospisil, S.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solar, M.; Solc, J.; Sopko, V.; Sopko, B.; Stekl, I.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Torregrosa, E. Fullana; Kodys, P.; Leitner, R.; Novakova, J.; Pleskot, V.; Rybar, M.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.; Wilhelm, I.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Ammosov, V. V.; Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Ivashin, A. V.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] Inst High Energy Phys, State Res Ctr, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Gillman, A. R.; Haywood, S. J.; Kirk, J.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Tyndel, M.; Wickens, F. J.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Benslama, K.] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Artoni, G.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Pedis, D.; De Salvo, A.; De Zorzi, G.; Dionisi, C.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Rossi, E.; Tehrani, F. Safai; Sidoti, A.; Camillocci, E. 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[Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Branchini, P.; Ceradini, F.; Di Luise, S.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Stanescu, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Luise, S.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.; Lablak, S.] Univ Hassan 2, Fac Sci Ain Chock, Reseau Univ Phys Hautes Energies, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA Marrakech, Oujda, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Abreu, H.; Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Bolnet, N. M.; Boonekamp, M.; Chevalier, L.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Grabas, H. M. X.; Guyot, C.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Legendre, M.; Maiani, C.; Mal, P.; Ramos, J. A. Manjarres; Mansoulie, B.; Martinez, H.; Meric, N.; Meyer, J-P.; Mijovic, L.; Hong, V. Nguyen Thi; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Resende, B.; Royon, C. R.; Salvatore, D.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.; Taffard, A.; Tsionou, D.; Vranjes, N.; Xiao, M.] CEA Saclay, DSM IRFU, F-91191 Gif Sur Yvette, France. [Damiani, D. S.; Grillo, A. A.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Mitrevski, J.; Nielsen, J.; Sadrozinski, W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Beckingham, M.; Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Hsu, S. -C.; Kaczmarska, A.; Keller, J. S.; Lubatti, H. J.; Rompotis, N.; Rothberg, J.; Verducci, M.; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Paredes, B. Lopez; Mcfayden, J. A.; Miyagawa, P. S.; Owen, S.; Paganis, E.; Suruliz, K.; Tovey, D. R.; Tua, A.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Ibragimov, I.; Ikematsu, K.; Jamin, D. O.; Rammes, M.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Dawe, E.; Godfrey, J.; Kvita, J.; O'Neil, D. C.; Petteni, M.; Stelzer, B.; Tanasijczuk, A. J.; Trottier-McDonald, M.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Mayes, J. Backus; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Hansson, P.; Kagan, M.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nelson, T. K.; Piacquadio, G.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Strauss, E.; Su, D.; Swiatlowski, M.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Batkova, L.; Blazek, T.; Federic, P.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Ferencei, J.; Kladiva, E.; Seman, M.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Carrillo-Montoya, G. D.; Leney, K. J. C.; Garcia, B. R. Mellado; Quayle, W. B.; Ruan, X.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Asman, B.; Bendtz, K.; Bessidskaia, O.; Bohm, C.; Clement, C.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Holmgren, S. O.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Papadelis, A.; Petridis, A.; Plucinski, P.; Silverstein, S. B.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Asman, B.; Bendtz, K.; Bessidskaia, O.; Clement, C.; Gellerstedt, K.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Petridis, A.; Plucinski, P.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Ahmad, A.; Arfaoui, S.; DeWilde, B.; Engelmann, R.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Puldon, D.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Ahmad, A.; Arfaoui, S.; DeWilde, B.; Engelmann, R.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Puldon, D.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Bartsch, V.; De Santo, A.; Martin-Haugh, S.; Potter, C. J.; Rose, A.; Salvatore, F.; Castillo, I. Santoyo; Sutton, M. R.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Bangert, A.; Black, C. W.; Cuthbert, C.; Jeng, G. -Y.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Waugh, A. T.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Chu, M. L.; Hou, S.; Lee, C. A.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; Mazini, R.; Ren, Z. L.; Soh, D. A.; Wang, J.; Wang, S. M.; Weng, Z.; Zhang, L.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Akimoto, G.; Di Mattia, A.; Hanawa, K.; Kajomovitz, E.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; Teng, P. K.; Vallecorsa, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Alhroob, M.; Amram, N.; Bella, G.; Benary, O.; Benhammou, Y.; Etzion, E.; Gershon, A.; Gueta, O.; Guttman, N.; Munwes, Y.; Oren, Y.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkialas, I.; Iliadis, D.; Kordas, K.; Kouskoura, V.; Nomidis, I.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Ishitsuka, M.; Jinnouchi, O.; Kanno, T.; Kuze, M.; Nagai, R.; Nobe, T.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Bailey, D. C.; Brelier, B.; Farooque, T.; Fatholahzadeh, B.; Ilic, N.; Keung, J.; Krieger, P.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Spreitzer, T.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Canepa, A.; Chekulaev, S. V.; Fortin, D.; Koutsman, A.; Oram, C. J.; Codina, E. Perez; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Bustos, A. C. Florez; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Kurata, M.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Napier, A.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Losty, M. J.; Loureiro, K. F.; Navas, L. Mendoza; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Gerbaudo, D.; Eschrich, I. Gough; Lankford, A. J.; Magnoni, L.; Mete, A. S.; Nelson, A.; Rao, K.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Toggerson, B.; Unel, G.; Werth, M.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Pinamonti, M.; Shaw, K.; Soualah, R.] Ist Nazl Fis Nucl, Grp Coll Udine, Udine, Italy. [Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Shaw, K.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Coggeshall, J.; Errede, D.; Errede, S.; Lie, K.; Liss, T. M.; McCarn, A.; Neubauer, M. S.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Brenner, R.; Buszello, C. P.; Coniavitis, E.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Pelikan, D.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] Univ Valencia, IFIC, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] Univ Valencia, IMB CNM, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] CSIC, Valencia, Spain. [Axen, D.; Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Loh, C. W.; Mills, W. J.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Astbury, A.; Bansal, V.; Berghaus, F.; Courneyea, L.; David, C.; Fincke-Keeler, M.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Lessard, J-R.; Marino, C. P.; Martyniuk, A. C.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Farrington, S. M.; Janus, M.; Jeske, C.; Jones, G.; Martin, T. A.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Kimura, N.; Mitani, T.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Alon, R.; Barak, L.; Bressler, S.; Citron, Z. H.; Duchovni, E.; Gabizon, O.; Gross, E.; Groth-Jensen, J.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Milstein, D.; Roth, I.; Silbert, O.; Smakhtin, V.; Vitells, O.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Castaneda-Miranda, E.; Chen, X.; Dos Anjos, A.; Castillo, L. R. Flores; Gutzwiller, O.; Hard, A. S.; Jared, R. C.; Ji, H.; Ju, X.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Morales, M. I. Pedraza; Sarangi, T.; Wang, H.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Fleischmann, P.; Redelbach, A.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Barisonzi, M.; Becker, K.; Becks, K. H.; Beermann, T. A.; Boek, J.; Boek, T. T.; Braun, H. M.; Cornelissen, T.; Duda, D.; Fischer, J.; Fleischmann, S.; Flick, T.; Gorfine, G.; Hamacher, K.; Harenberg, T.; Hirschbuehl, D.; Kalinin, S.; Kersten, S.; Khoroshilov, A.; Kohlmann, S.; Lenzen, G.; Maettig, P.; Mechtel, M.; Neumann, M.; Pataraia, S.; Sandhoff, M.; Sartisohn, G.; Sturm, P.; Wagner, W.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany. [Adelman, J.; Baker, O. K.; Bedikian, S.; Almenar, C. Cuenca; Cummings, J.; Czyczula, Z.; Demers, S.; Erdmann, J.; Garberson, F.; Golling, T.; Guest, D.; Henrichs, A.; Lagouri, T.; Lee, L.; Leister, A. G.; Loginov, A.; Tipton, P.; Wall, R.; Walsh, B.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Bernlochner, F. U.; Hakobyan, H.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] Inst Natl Phys Nucl & Phys Particules, Ctr Calcul, IN2P3, Villeurbanne, France. [Acharya, B. S.] Kings Coll London, Dept Phys, London, England. [Amorim, A.; Gomes, A.; Maio, A.; Pina, J.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amorim, A.; Gomes, A.; Maio, A.; Pina, J.] Univ Lisbon, CFNUL, Lisbon, Portugal. [Bawa, H. S.; Gao, Y. S.; Lowe, A. J.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beloborodova, O. L.; Maximov, D. A.; Talyshev, A. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Carvalho, J.; Fiolhais, M. C. N.; Oliveira, M.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Demirkoz, B.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Dhullipudi, R.; Greenwood, Z. D.; Sawyer, L.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Wemans, A. Do Valle] Univ Nova Lisboa, Dep Fis, Caparica, Portugal. [Wemans, A. Do Valle] Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Gkialas, I.; Papageorgiou, K.] Univ Aegean, Dept Financial & Management Engn, Chios, Greece. [Grinstein, S.; Rozas, A. Juste; Martinez, M.] ICREA, Barcelona, Spain. [Kono, T.; Wildt, M. A.] Univ Hamburg, Inst Expt Phys, Hamburg, Germany. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Liang, Z.; Soh, D. A.; Weng, Z.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou, Peoples R China. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Mal, P.] Natl Inst Sci Educ & Res, Sch Phys Sci, Bhubaneswar, Orissa, India. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Nessi, M.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Pasztor, G.; Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Pinamonti, M.] SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Tamsett, M. C.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Vickey, T.] Univ Oxford, Dept Phys, Oxford, England. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. [Acharya, B. S.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] Univ Paris Diderot, Paris, France. RP Aad, G (reprint author), Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. RI Doyle, Anthony/C-5889-2009; Ferrando, James/A-9192-2012; Solfaroli Camillocci, Elena/J-1596-2012; Lee, Jason/B-9701-2014; Robson, Aidan/G-1087-2011; Kuday, Sinan/C-8528-2014; Snesarev, Andrey/H-5090-2013; Warburton, Andreas/N-8028-2013; Turchikhin, Semen/O-1929-2013; Boyko, Igor/J-3659-2013; Smirnova, Oxana/A-4401-2013; Sukharev, Andrey/A-6470-2014; Gabrielli, Alessandro/H-4931-2012; Zimmermann, Claus/E-9598-2014; Fabbri, Laura/H-3442-2012; Brooks, William/C-8636-2013; Villa, Mauro/C-9883-2009; Nozka, Libor/G-5550-2014; Nemecek, Stanislav/G-5931-2014; Kepka, Oldrich/G-6375-2014; Lokajicek, Milos/G-7800-2014; Jakoubek, Tomas/G-8644-2014; Staroba, Pavel/G-8850-2014; Kupco, Alexander/G-9713-2014; de Groot, Nicolo/A-2675-2009; Hejbal, Jiri/H-1358-2014; Marcisovsky, Michal/H-1533-2014; Mikestikova, Marcela/H-1996-2014; Lysak, Roman/H-2995-2014; Tomasek, Lukas/G-6370-2014; Svatos, Michal/G-8437-2014; Chudoba, Jiri/G-7737-2014; Moraes, Arthur/F-6478-2010; Peleganchuk, Sergey/J-6722-2014; Bosman, Martine/J-9917-2014; Castro, Nuno/D-5260-2011; Grinstein, Sebastian/N-3988-2014; Wemans, Andre/A-6738-2012; Gutierrez, Phillip/C-1161-2011; Ventura, Andrea/A-9544-2015; Livan, Michele/D-7531-2012; De, Kaushik/N-1953-2013; Mitsou, Vasiliki/D-1967-2009; White, Ryan/E-2979-2015; Joergensen, Morten/E-6847-2015; Riu, Imma/L-7385-2014; Mir, Lluisa-Maria/G-7212-2015; Della Pietra, Massimo/J-5008-2012; Cavalli-Sforza, Matteo/H-7102-2015; Petrucci, Fabrizio/G-8348-2012; Negrini, Matteo/C-8906-2014; Ferrer, Antonio/H-2942-2015; Hansen, John/B-9058-2015; Grancagnolo, Sergio/J-3957-2015; spagnolo, stefania/A-6359-2012; Ciubancan, Liviu Mihai/L-2412-2015; Shmeleva, Alevtina/M-6199-2015; Camarri, Paolo/M-7979-2015; Gavrilenko, Igor/M-8260-2015; Akimov, Andrey/N-1769-2015; Tikhomirov, Vladimir/M-6194-2015; Chekulaev, Sergey/O-1145-2015; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; Andreazza, Attilio/E-5642-2011; Carvalho, Joao/M-4060-2013; Demirkoz, Bilge/C-8179-2014; Mashinistov, Ruslan/M-8356-2015; Buttar, Craig/D-3706-2011; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Olshevskiy, Alexander/I-1580-2016; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Mora Herrera, Maria Clemencia/L-3893-2016; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; KHODINOV, ALEKSANDR/D-6269-2015; Gauzzi, Paolo/D-2615-2009; O'Shea, Val/G-1279-2010; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Yang, Haijun/O-1055-2015; Monzani, Simone/D-6328-2017; Grancagnolo, Francesco/K-2857-2015; Korol, Aleksandr/A-6244-2014; Karyukhin, Andrey/J-3904-2014; Capua, Marcella/A-8549-2015; Tartarelli, Giuseppe Francesco/A-5629-2016; McKee, Shawn/B-6435-2012; Fassi, Farida/F-3571-2016; la rotonda, laura/B-4028-2016; OI Doyle, Anthony/0000-0001-6322-6195; Ferrando, James/0000-0002-1007-7816; Solfaroli Camillocci, Elena/0000-0002-5347-7764; Lee, Jason/0000-0002-2153-1519; Kuday, Sinan/0000-0002-0116-5494; Warburton, Andreas/0000-0002-2298-7315; Turchikhin, Semen/0000-0001-6506-3123; Boyko, Igor/0000-0002-3355-4662; Smirnova, Oxana/0000-0003-2517-531X; Gabrielli, Alessandro/0000-0001-5346-7841; Fabbri, Laura/0000-0002-4002-8353; Brooks, William/0000-0001-6161-3570; Villa, Mauro/0000-0002-9181-8048; Mikestikova, Marcela/0000-0003-1277-2596; Tomasek, Lukas/0000-0002-5224-1936; Svatos, Michal/0000-0002-7199-3383; Moraes, Arthur/0000-0002-5157-5686; Peleganchuk, Sergey/0000-0003-0907-7592; Bosman, Martine/0000-0002-7290-643X; Castro, Nuno/0000-0001-8491-4376; Grinstein, Sebastian/0000-0002-6460-8694; Wemans, Andre/0000-0002-9669-9500; Ventura, Andrea/0000-0002-3368-3413; Livan, Michele/0000-0002-5877-0062; De, Kaushik/0000-0002-5647-4489; Mitsou, Vasiliki/0000-0002-1533-8886; White, Ryan/0000-0003-3589-5900; Joergensen, Morten/0000-0002-6790-9361; Riu, Imma/0000-0002-3742-4582; Mir, Lluisa-Maria/0000-0002-4276-715X; Della Pietra, Massimo/0000-0003-4446-3368; Petrucci, Fabrizio/0000-0002-5278-2206; Negrini, Matteo/0000-0003-0101-6963; Ferrer, Antonio/0000-0003-0532-711X; Hansen, John/0000-0002-8422-5543; Grancagnolo, Sergio/0000-0001-8490-8304; spagnolo, stefania/0000-0001-7482-6348; Ciubancan, Liviu Mihai/0000-0003-1837-2841; Camarri, Paolo/0000-0002-5732-5645; Tikhomirov, Vladimir/0000-0002-9634-0581; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; Andreazza, Attilio/0000-0001-5161-5759; Carvalho, Joao/0000-0002-3015-7821; Mashinistov, Ruslan/0000-0001-7925-4676; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Vykydal, Zdenek/0000-0003-2329-0672; Olshevskiy, Alexander/0000-0002-8902-1793; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Gauzzi, Paolo/0000-0003-4841-5822; O'Shea, Val/0000-0001-7183-1205; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Monzani, Simone/0000-0002-0479-2207; Grancagnolo, Francesco/0000-0002-9367-3380; Korol, Aleksandr/0000-0001-8448-218X; Karyukhin, Andrey/0000-0001-9087-4315; Smestad, Lillian/0000-0002-0244-8736; Giordani, Mario/0000-0002-0792-6039; Capua, Marcella/0000-0002-2443-6525; Di Micco, Biagio/0000-0002-4067-1592; Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; McKee, Shawn/0000-0002-4551-4502; Doria, Alessandra/0000-0002-5381-2649; Veloso, Filipe/0000-0002-5956-4244; Fassi, Farida/0000-0002-6423-7213; la rotonda, laura/0000-0002-6780-5829; Osculati, Bianca Maria/0000-0002-7246-060X; Amorim, Antonio/0000-0003-0638-2321; Coccaro, Andrea/0000-0003-2368-4559 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF; DNSRC; Lundbeck Foundation, Denmark; EPLANET; ERC; NSRF; European Union; IN2P3-CNRS; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF; DFG; HGF; MPG; AvH Foundation, Germany FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; ISF, MINERVA, GIF, DIP and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW, Poland; GRICES and FCT, Portugal; MERYS (MECTS), Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZ. S, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America.; The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 77 TC 37 Z9 37 U1 7 U2 150 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD OCT 29 PY 2013 IS 10 AR 189 DI 10.1007/JHEP10(2013)189 PG 40 WC Physics, Particles & Fields SC Physics GA 243DM UT WOS:000326296900004 ER PT J AU Davis, JCS Lee, DH AF Davis, J. C. Seamus Lee, Dung-Hai TI Concepts relating magnetic interactions, intertwined electronic orders, and strongly correlated superconductivity SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE high-Tc superconductivity; strong correlations; fermiology ID HIGH-TEMPERATURE SUPERCONDUCTIVITY; VALENCE BOND STATE; T-C SUPERCONDUCTOR; CUPRATE SUPERCONDUCTORS; PSEUDOGAP STATE; PHYSICS; INSTABILITY; TRANSITION; COMPLEXITY; ANISOTROPY AB Unconventional superconductivity (SC) is said to occur when Cooper pair formation is dominated by repulsive electron-electron interactions, so that the symmetry of the pair wave function is other than an isotropic s-wave. The strong, on-site, repulsive electron-electron interactions that are the proximate cause of such SC are more typically drivers of commensurate magnetism. Indeed, it is the suppression of commensurate antiferromagnetism (AF) that usually allows this type of unconventional superconductivity to emerge. Importantly, however, intervening between these AF and SC phases, intertwined electronic ordered phases (IP) of an unexpected nature are frequently discovered. For this reason, it has been extremely difficult to distinguish the microscopic essence of the correlated superconductivity from the often spectacular phenomenology of the IPs. Here we introduce a model conceptual framework within which to understand the relationship between AF electron-electron interactions, IPs, and correlated SC. We demonstrate its effectiveness in simultaneously explaining the consequences of AF interactions for the copper-based, iron-based, and heavy-fermion superconductors, as well as for their quite distinct IPs. C1 [Davis, J. C. Seamus] Cornell Univ, Dept Phys, Ithaca, NY 14853 USA. [Davis, J. C. Seamus] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Davis, J. C. Seamus] Univ St Andrews, Sch Phys & Astron, St Andrews KY16 9SS, Fife, Scotland. [Davis, J. C. Seamus] Cornell Univ, Kavli Inst Cornell Nanoscale Sci, Ithaca, NY 14853 USA. [Lee, Dung-Hai] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Lee, Dung-Hai] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Davis, JCS (reprint author), Cornell Univ, Dept Phys, Ithaca, NY 14853 USA. EM jcdavis@ccmr.cornell.edu; dunghai@berkeley.edu FU US Department of Energy (DOE) [Grant DE-2009-BNL-PM015]; DOE Office of Basic Energy Sciences, Division of Materials Science [DE-AC02-05CH11231]; Center for Emergent Superconductivity, an Energy Frontier Research Center; Energy Frontier Research Center at Brookhaven National Laboratory FX We thank S. A. Kivelson for a most useful discussion on the Q = 0 instabilities in the cuprates. We also thank D. K. Morr, M. Norman, and S. Sachdev for helpful discussions and communications. J.C.S.D. is supported by the Center for Emergent Superconductivity, an Energy Frontier Research Center, headquartered at Brookhaven National Laboratory and funded by the US Department of Energy (DOE), under Grant DE-2009-BNL-PM015. D.-H.L. is supported by the DOE Office of Basic Energy Sciences, Division of Materials Science, under Grant DE-AC02-05CH11231. NR 59 TC 70 Z9 70 U1 6 U2 37 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD OCT 29 PY 2013 VL 110 IS 44 BP 17623 EP 17630 DI 10.1073/pnas.1316512110 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 242LJ UT WOS:000326243100019 PM 24114268 ER PT J AU Chakraborty, S Jackson, TL Ahmed, M Thiemens, MH AF Chakraborty, Subrata Jackson, Teresa L. Ahmed, Musahid Thiemens, Mark H. TI Sulfur isotopic fractionation in vacuum UV photodissociation of hydrogen sulfide and its potential relevance to meteorite analysis SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE chondrites; achondrites; isotope ID MULTIPHOTON IONIZATION SPECTROSCOPY; MASS-INDEPENDENT FRACTIONATION; SOLAR NEBULA; CARBONACEOUS CHONDRITES; NO2 ISOTOPOLOGUES; H2S MOLECULE; OXYGEN; SYSTEM; DYNAMICS; DISSOCIATION AB Select meteoritic classes possess mass-independent sulfur isotopic compositions in sulfide and organic phases. Photochemistry in the solar nebula has been attributed as a source of these anomalies. Hydrogen sulfide (H2S) is the most abundant gas-phase species in the solar nebula, and hence, photodissociation of H2S by solar vacuum UV (VUV) photons (especially by Lyman-alpha radiation) is a relevant process. Because of experimental difficulties associated with accessing VUV radiation, there is a paucity of data and a lack of theoretical basis to test the hypothesis of a photochemical origin of mass-independent sulfur. Here, we present multiisotopic measurements of elemental sulfur produced during the VUV photolysis of H2S. Mass-independent sulfur isotopic compositions are observed. The observed isotopic fractionation patterns are wavelength-dependent. VUV photodissociation of H2S takes place through several predissociative channels, and the measured mass-independent fractionation is most likely a manifestation of these processes. Meteorite sulfur data are discussed in light of the present experiments, and suggestions are made to guide future experiments and models. C1 [Chakraborty, Subrata; Jackson, Teresa L.; Thiemens, Mark H.] Univ Calif San Diego, Dept Chem & Biochem, La Jolla, CA 92093 USA. [Ahmed, Musahid] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Chakraborty, S (reprint author), Univ Calif San Diego, Dept Chem & Biochem, La Jolla, CA 92093 USA. EM s1chakraborty@ucsd.edu RI Ahmed, Musahid/A-8733-2009 FU Office of Science, Office of Basic Energy Sciences; Division of Chemical Sciences, Geosciences, and Biosciences of the US Department of Energy at Lawrence Berkeley National Laboratory [DE-AC02-05CH11231] FX S. C. thanks Ryan D. Davis for his help in performing experiments at Advanced Light Source. Support from Ms. Sarah Ferrell and Dr. Amir Golan (Chemical Dynamics Beamline at the Advanced Light Source) and Dr. Doug Taube (Chemistry Laboratory Manager of Advanced Light Source) is acknowledged. Two anonymous reviewers and the editor are acknowledged for comments that improved the manuscript. The work is funded through National Aeronautics and Space Administration's Origins and Cosmochemistry programs. M. A. and the Advanced Light Source are supported by the Director, Office of Science, Office of Basic Energy Sciences and the Division of Chemical Sciences, Geosciences, and Biosciences of the US Department of Energy at Lawrence Berkeley National Laboratory under Contract DE-AC02-05CH11231. NR 68 TC 6 Z9 6 U1 4 U2 29 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD OCT 29 PY 2013 VL 110 IS 44 BP 17650 EP 17655 DI 10.1073/pnas.1213150110 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 242LJ UT WOS:000326243100023 PM 23431159 ER PT J AU Fan, Y Osetskiy, YN Yip, S Yildiz, B AF Fan, Yue Osetskiy, Yuri N. Yip, Sidney Yildiz, Bilge TI Mapping strain rate dependence of dislocation-defect interactions by atomistic simulations SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE structural materials; mechanical properties; low strain rate atomistic simulation ID STACKING-FAULT TETRAHEDRON; MOLECULAR-DYNAMICS SIMULATIONS; IRRADIATED ZIRCONIUM ALLOYS; ALPHA-ZIRCONIUM; OBSTACLE INTERACTIONS; EDGE DISLOCATIONS; DEFORMATION; METALS; SCALE; MECHANISMS AB Probing the mechanisms of defect-defect interactions at strain rates lower than 10(6) s(-1) is an unresolved challenge to date to molecular dynamics (MD) techniques. Here we propose an original atomistic approach based on transition state theory and the concept of a strain-dependent effective activation barrier that is capable of simulating the kinetics of dislocation-defect interactions at virtually any strain rate, exemplified within 10(-7) to 10(7) s(-1). We apply this approach to the problem of an edge dislocation colliding with a cluster of self-interstitial atoms (SIAs) under shear deformation. Using an activation-relaxation algorithm [Kushima A, et al. (2009) J Chem Phys 130:224504], we uncover a unique strain-rate-dependent trigger mechanism that allows the SIA cluster to be absorbed during the process, leading to dislocation climb. Guided by this finding, we determine the activation barrier of the trigger mechanism as a function of shear strain, and use that in a coarse-graining rate equation formulation for constructing a mechanism map in the phase space of strain rate and temperature. Our predictions of a crossover from a defect recovery at the low strain-rate regime to defect absorption behavior in the high strain-rate regime are validated against our own independent, direct MD simulations at 10(5) to 10(7) s(-1). Implications of the present approach for probing molecular-level mechanisms in strain-rate regimes previously considered inaccessible to atomistic simulations are discussed. C1 [Fan, Yue; Yip, Sidney; Yildiz, Bilge] MIT, Dept Nucl Sci & Engn, Cambridge, MA 02139 USA. [Yip, Sidney] MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA. [Osetskiy, Yuri N.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Yildiz, B (reprint author), MIT, Dept Nucl Sci & Engn, 77 Massachusetts Ave, Cambridge, MA 02139 USA. EM byildiz@mit.edu RI FAN, YUE/H-1737-2011; OI Osetskiy, Yury/0000-0002-8109-0030 FU Consortium for Advanced Simulation of Light Water Reactors; Energy Innovation Hub for Modeling and Simulation of Nuclear Reactors under US Department of Energy [DE-AC05-00OR22725]; Division of Materials Sciences and Engineering, US Department of Energy FX This work was supported by the Consortium for Advanced Simulation of Light Water Reactors, an Energy Innovation Hub for Modeling and Simulation of Nuclear Reactors under US Department of Energy Contract DE-AC05-00OR22725, and Y.N.O. was supported by the Division of Materials Sciences and Engineering, US Department of Energy. NR 50 TC 28 Z9 28 U1 5 U2 55 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD OCT 29 PY 2013 VL 110 IS 44 BP 17756 EP 17761 DI 10.1073/pnas.1310036110 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 242LJ UT WOS:000326243100041 PM 24114271 ER PT J AU Zhao, JJ Chatterjee, U Ai, DF Hinks, DG Zheng, H Gu, GD Castellan, JP Rosenkranz, S Claus, H Norman, MR Randeria, M Campuzano, JC AF Zhao, Junjing Chatterjee, Utpal Ai, Dingfei Hinks, David G. Zheng, Hong Gu, G. D. Castellan, John-Paul Rosenkranz, Stephan Claus, Helmut Norman, Michael R. Randeria, Mohit Campuzano, Juan Carlos TI Universal features in the photoemission spectroscopy of high-temperature superconductors SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article ID T-C SUPERCONDUCTOR; UNDERDOPED BI2SR2CACU2O8+DELTA; QUASI-PARTICLES; GAP ANISOTROPY; NORMAL-STATE; ENERGY GAPS; PSEUDOGAP; SYMMETRY AB The energy gap for electronic excitations is one of the most important characteristics of the superconducting state, as it directly reflects the pairing of electrons. In the copper-oxide high-temperature superconductors (HTSCs), a strongly anisotropic energy gap, which vanishes along high-symmetry directions, is a clear manifestation of the d-wave symmetry of the pairing. There is, however, a dramatic change in the form of the gap anisotropy with reduced carrier concentration (underdoping). Although the vanishing of the gap along the diagonal to the square Cu-O bond directions is robust, the doping dependence of the large gap along the Cu-O directions suggests that its origin might be different from pairing. It is thus tempting to associate the large gap with a second-order parameter distinct from superconductivity. We use angle-resolved photoemission spectroscopy to show that the two-gap behavior and the destruction of well-defined electronic excitations are not universal features of HTSCs, and depend sensitively on how the underdoped materials are prepared. Depending on cation substitution, underdoped samples either show two-gap behavior or not. In contrast, many other characteristics of HTSCs, such as the dome-like dependence of T-c on doping, long-lived excitations along the diagonals to the Cu-O bonds, and an energy gap at the Brillouin zone boundary that decreases monotonically with doping while persisting above T-c (the pseudogap), are present in all samples, irrespective of whether they exhibit two-gap behavior or not. Our results imply that universal aspects of high-T-c superconductivity are relatively insensitive to differences in the electronic states along the Cu-O bond directions. C1 [Zhao, Junjing; Ai, Dingfei; Campuzano, Juan Carlos] Univ Illinois, Dept Phys, Chicago, IL 60607 USA. [Zhao, Junjing; Chatterjee, Utpal; Hinks, David G.; Zheng, Hong; Castellan, John-Paul; Rosenkranz, Stephan; Claus, Helmut; Norman, Michael R.; Campuzano, Juan Carlos] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Gu, G. D.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Randeria, Mohit] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. RP Campuzano, JC (reprint author), Univ Illinois, Dept Phys, Chicago, IL 60607 USA. EM jcc@uic.edu RI Rosenkranz, Stephan/E-4672-2011; Norman, Michael/C-3644-2013 OI Rosenkranz, Stephan/0000-0002-5659-0383; FU Basic Energy Sciences (BES), Office of Science, US Department of Energy (DOE) [DE-AC02-06CH11357]; DOE-BES [DE-SC0005035]; DOE [DE-AC02-98CH10886]; University of Wisconsin-Madison FX We thank D. Robinson and J.P.C. Ruff for support with the high-energy X-ray diffraction measurements. Work at Argonne was supported by Basic Energy Sciences (BES), Office of Science, US Department of Energy (DOE) under Contract DE-AC02-06CH11357 (to J.Z., U.C., D.G. H., H.Z., S.R., H.C., M.R.N., and J.C.C.). M.R. was supported by the DOE-BES Grant DE-SC0005035. G.D.G. was supported by the DOE Contract No. DE-AC02-98CH10886. The Synchrotron Radiation Center is supported by the University of Wisconsin-Madison. NR 31 TC 5 Z9 5 U1 4 U2 19 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD OCT 29 PY 2013 VL 110 IS 44 BP 17774 EP 17777 DI 10.1073/pnas.1302932110 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 242LJ UT WOS:000326243100044 PM 24101464 ER PT J AU Edayathumangalam, R Wu, R Garcia, R Wang, YG Wang, W Kreinbring, CA Bach, A Liao, JL Stone, TA Terwilliger, TC Hoang, QQ Belitsky, BR Petsko, GA Ringe, D Liu, D AF Edayathumangalam, Raji Wu, Rui Garcia, Roman Wang, Yuguang Wang, Wei Kreinbring, Cheryl A. Bach, Alicia Liao, Jingling Stone, Todd A. Terwilliger, Thomas C. Hoang, Quyen Q. Belitsky, Boris R. Petsko, Gregory A. Ringe, Dagmar Liu, Dali TI Crystal structure of Bacillus subtilis GabR, an autorepressor and transcriptional activator of gabT SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article ID ASPARTATE-AMINOTRANSFERASE; DEPENDENT ENZYMES; FACTOR FADR; PROTEIN; DOMAINS; RECOGNITION; BINDING; FAMILY; MOCR AB Bacillus subtilis GabR is a transcription factor that regulates gamma-aminobutyric acid (GABA) metabolism. GabR is a member of the understudied MocR/GabR subfamily of the GntR family of transcription regulators. A typical MocR/GabR-type regulator is a chimeric protein containing a short N-terminal helix-turn-helix DNA-binding domain and a long C-terminal pyridoxal 5'-phosphate (PLP)-binding putative aminotransferase domain. In the presence of PLP and GABA, GabR activates the gabTD operon, which allows the bacterium to use GABA as nitrogen and carbon sources. GabR binds to its own promoter and represses gabR transcription in the absence of GABA. Here, we report two crystal structures of full-length GabR from B. subtilis: a 2.7-angstrom structure of GabR with PLP bound and the 2.55-angstrom apo structure of GabR without PLP. The quaternary structure of GabR is a head-to-tail domain-swap homodimer. Each monomer comprises two domains: an N-terminal winged-helix DNA-binding domain and a C-terminal PLP-binding type I aminotransferase-like domain. The winged-helix domain contains putative DNA-binding residues conserved in other GntR-type regulators. Together with sedimentation velocity and fluorescence polarization assays, the crystal structure of GabR provides insights into DNA binding by GabR at the gabR and gabT promoters. The absence of GabR-mediated aminotransferase activity in the presence of GABA and PLP, and the presence of an active site configuration that is incompatible with stabilization of the GABA external aldimine suggest that a GabR aminotransferase-like activity involving GABA and PLP is not essential to its primary function as a transcription regulator. C1 [Edayathumangalam, Raji] Harvard Univ, Sch Med, Ctr Neurol Dis, Boston, MA 02115 USA. [Edayathumangalam, Raji] Brigham & Womens Hosp, Boston, MA 02115 USA. [Edayathumangalam, Raji; Kreinbring, Cheryl A.; Bach, Alicia; Petsko, Gregory A.; Ringe, Dagmar] Brandeis Univ, Rosenstiel Basic Med Sci Res Ctr, Dept Biochem, Waltham, MA 02454 USA. [Wu, Rui; Garcia, Roman; Wang, Yuguang; Liu, Dali] Loyola Univ, Dept Chem & Biochem, Chicago, IL 60626 USA. [Wang, Wei; Liao, Jingling; Hoang, Quyen Q.] Indiana Univ, Sch Med, Stark Neurosci Res Inst, Dept Biochem & Mol Biol, Indianapolis, IN 46202 USA. [Stone, Todd A.] Indiana Univ, Dept Mol & Cellular Biochem, Bloomington, IN 47405 USA. [Terwilliger, Thomas C.] Los Alamos Natl Lab, Biosci Div, Los Alamos, NM 87545 USA. [Belitsky, Boris R.] Tufts Univ, Sch Med, Dept Mol Biol & Microbiol, Boston, MA 02111 USA. RP Petsko, GA (reprint author), Brandeis Univ, Rosenstiel Basic Med Sci Res Ctr, Dept Biochem, Waltham, MA 02454 USA. EM petsko@brandeis.edu; ringe@brandeis.edu; dliu@luc.edu RI Terwilliger, Thomas/K-4109-2012 OI Terwilliger, Thomas/0000-0001-6384-0320 FU Loyola University Chicago; NSF [CHE-1308672, MCB-0110651]; National Institutes of Health FX We thank Boguslaw Nocek (Structural Biology Center, Sector 19) at Advance Photon Source, Argonne National Laboratory for help with data collection; Zbyszek Dauter, Eleanor Dodson, Frank DiMaio, Nathaniel Echols, Julia Klutkowski, Ruslan Sanishvili, Miguel Ballicora, and Janet Smith for helpful discussions, suggestions, and/or technical help. This work was funded by the start-up funds from Loyola University Chicago (to D.L.), an NSF subaward from Grant CHE-1308672 (to D.L.), NSF Grant MCB-0110651 (to B.R.B.), and a grant from the National Institutes of Health (to D.R. and G.A.P.). NR 19 TC 23 Z9 23 U1 2 U2 10 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD OCT 29 PY 2013 VL 110 IS 44 BP 17820 EP 17825 DI 10.1073/pnas.1315887110 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 242LJ UT WOS:000326243100052 PM 24127574 ER PT J AU Parker, SCJ Stitzel, ML Taylor, DL Orozco, JM Erdos, MR Akiyama, JA van Bueren, KL Chines, PS Narisu, N Black, BL Visel, A Pennacchio, LA Collins, FS AF Parker, Stephen C. J. Stitzel, Michael L. Taylor, D. Leland Orozco, Jose Miguel Erdos, Michael R. Akiyama, Jennifer A. van Bueren, Kelly Lammerts Chines, Peter S. Narisu, Narisu Black, Brian L. Visel, Axel Pennacchio, Len A. Collins, Francis S. CA NISC Comparative Sequencing TI Chromatin stretch enhancer states drive cell-specific gene regulation and harbor human disease risk variants SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article ID SUPER-ENHANCERS; SNP RS6983267; HUMAN GENOME; DISCOVERY; ELEMENTS; DNA; ANNOTATION; EXPRESSION; COHESIN; ISLETS AB Chromatin-based functional genomic analyses and genomewide association studies (GWASs) together implicate enhancers as critical elements influencing gene expression and risk for common diseases. Here, we performed systematic chromatin and transcriptome profiling in human pancreatic islets. Integrated analysis of islet data with those from nine cell types identified specific and significant enrichment of type 2 diabetes and related quantitative trait GWAS variants in islet enhancers. Our integrated chromatin maps reveal that most enhancers are short (median = 0.8 kb). Each cell type also contains a substantial number of more extended (>= 3 kb) enhancers. Interestingly, these stretch enhancers are often tissue-specific and overlap locus control regions, suggesting that they are important chromatin regulatory beacons. Indeed, we show that (i) tissue specificity of enhancers and nearby gene expression increase with enhancer length; (ii) neighborhoods containing stretch enhancers are enriched for important cell type-specific genes; and (iii) GWAS variants associated with traits relevant to a particular cell type are more enriched in stretch enhancers compared with short enhancers. Reporter constructs containing stretch enhancer sequences exhibited tissue-specific activity in cell culture experiments and in transgenic mice. These results suggest that stretch enhancers are critical chromatin elements for coordinating cell type-specific regulatory programs and that sequence variation in stretch enhancers affects risk of major common human diseases. C1 [Parker, Stephen C. J.; Stitzel, Michael L.; Taylor, D. Leland; Orozco, Jose Miguel; Erdos, Michael R.; Chines, Peter S.; Narisu, Narisu; Collins, Francis S.; NISC Comparative Sequencing] Natl Human Genome Res Inst, NIH, Bethesda, MD 20892 USA. [Akiyama, Jennifer A.; Visel, Axel; Pennacchio, Len A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Genom Div, Berkeley, CA 94720 USA. [van Bueren, Kelly Lammerts; Black, Brian L.] Univ Calif San Francisco, Cardiovasc Res Inst, San Francisco, CA 95158 USA. [Visel, Axel; Pennacchio, Len A.] Joint Genome Inst, Dept Energy, Walnut Creek, CA 94598 USA. RP Collins, FS (reprint author), Natl Human Genome Res Inst, NIH, Bethesda, MD 20892 USA. EM collinsf@od.nih.gov RI Visel, Axel/A-9398-2009; OI Visel, Axel/0000-0002-4130-7784; Black, Brian/0000-0002-6664-8913; Taylor, Leland/0000-0001-6498-6970 FU Postdoctoral Research Associate (PRAT) fellowship [1ZIAHG000024, K99DK092251, K99DK099240, R01HL64658, R01DE019118]; E.O. Lawrence Berkeley National Laboratory [R01HG003988]; Department of Energy, University of California [DEAC02-05CH11231] FX We thank the Finland United States Investigation of NIDDM Genetics Consortium and National Institutes of Health (NIH) Chromatin community for valuable critiques and discussion. We thank Lori Bonnycastle, Laura Elnitski, Andrea Ramirez, Mario Morken, and Adam Woolfe for helpful comments. Human islets were obtained from organ donors through the ICR Basic Science Islet Distribution Program (Universities of Illinois, Washington, Miami, and Alabama at Birmingham) and the National Disease Research Interchange. We thank the reviewers for excellent feedback and suggestions. This work was supported by Postdoctoral Research Associate (PRAT) fellowship (to S.C.J.P.); Grants 1ZIAHG000024 (to F.S.C.), K99DK092251 (to M.L.S.), K99DK099240 (to S.C.J.P.), R01HL64658 (to B.L.B.), and R01DE019118 (to B.L.B.). A.V. and L.A.P. are supported by Grant R01HG003988 and conducted research at the E.O. Lawrence Berkeley National Laboratory, performed under Department of Energy Contract DEAC02-05CH11231, University of California. NR 33 TC 150 Z9 150 U1 2 U2 23 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD OCT 29 PY 2013 VL 110 IS 44 BP 17921 EP 17926 DI 10.1073/pnas.1317023110 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 242LJ UT WOS:000326243100069 PM 24127591 ER PT J AU Chung, M Collura, MG Flanagan, G Freemire, B Hanlet, PM Jana, MR Johnson, RP Kaplan, DM Leonova, M Moretti, A Popovic, M Schwarz, T Tollestrup, A Torun, Y Yonehara, K AF Chung, M. Collura, M. G. Flanagan, G. Freemire, B. Hanlet, P. M. Jana, M. R. Johnson, R. P. Kaplan, D. M. Leonova, M. Moretti, A. Popovic, M. Schwarz, T. Tollestrup, A. Torun, Y. Yonehara, K. TI Pressurized H-2 rf Cavities in Ionizing Beams and Magnetic Fields SO PHYSICAL REVIEW LETTERS LA English DT Article ID HYDROGEN; ELECTRONS; GASES; IONS AB A major technological challenge in building a muon cooling channel is operating rf cavities in multitesla external magnetic fields. We report the first proof-of-principle experiment of a high pressure gas-filled rf cavity for use with intense ionizing beams and strong external magnetic fields. rf power consumption by beam-induced plasma is investigated with hydrogen and deuterium gases with pressures between 20 and 100 atm and peak rf gradients between 5 and 50 MV/m. The low pressure case agrees well with an analytical model based on electron and ion mobilities. Varying concentrations of oxygen gas are investigated to remove free electrons from the cavity and reduce the rf power consumption. Measurements of the electron attachment time to oxygen and rate of ion-ion recombination are also made. Additionally, we demonstrate the operation of the gas-filled rf cavity in a solenoidal field of up to 3 T, finding no major magnetic field dependence. All these results indicate that a high pressure gas-filled cavity is a viable technology for muon ionization cooling. C1 [Chung, M.; Collura, M. G.; Jana, M. R.; Leonova, M.; Moretti, A.; Popovic, M.; Schwarz, T.; Tollestrup, A.; Yonehara, K.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Flanagan, G.; Johnson, R. P.] Muons Inc, Batavia, IL 60134 USA. [Freemire, B.; Hanlet, P. M.; Kaplan, D. M.; Torun, Y.] IIT, Chicago, IL 60616 USA. RP Chung, M (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. FU Fermi Research Alliance, LLC [DE-AC02-07CH11359]; U.S. Department of Energy; U.S. Department of Energy STTR [DE-C00006266]; U.S. Muon Accelerator Program (MAP) FX The authors would like to thank R. Johnsen (University of Pittsburgh) for helpful comments and discussions. Fermilab is operated by Fermi Research Alliance, LLC under Contract No. DE-AC02-07CH11359 with the U.S. Department of Energy. This work was partially supported by U.S. Department of Energy STTR Grant No. DE-C00006266 and by grants from the U.S. Muon Accelerator Program (MAP) to Illinois Institute of Technology. NR 30 TC 4 Z9 4 U1 0 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 29 PY 2013 VL 111 IS 18 AR 184802 DI 10.1103/PhysRevLett.111.184802 PG 5 WC Physics, Multidisciplinary SC Physics GA 242XM UT WOS:000326279100012 PM 24237526 ER PT J AU Hay, MJ Valeo, EJ Fisch, NJ AF Hay, Michael J. Valeo, Ernest J. Fisch, Nathaniel J. TI Geometrical Optics of Dense Aerosols: Forming Dense Plasma Slabs SO PHYSICAL REVIEW LETTERS LA English DT Article ID EXPANSIONS; BEAMS AB Assembling a freestanding, sharp-edged slab of homogeneous material that is much denser than gas, but much more rarefied than a solid, is an outstanding technological challenge. The solution may lie in focusing a dense aerosol to assume this geometry. However, whereas the geometrical optics of dilute aerosols is a well-developed field, the dense aerosol limit is mostly unexplored. Yet controlling the geometrical optics of dense aerosols is necessary in preparing such a material slab. Focusing dense aerosols is shown here to be possible, but the finite particle density reduces the effective Stokes number of the flow, a critical result for controlled focusing. C1 [Hay, Michael J.; Fisch, Nathaniel J.] Princeton Univ, Dept Astrophys Sci, Princeton, NJ 08544 USA. [Valeo, Ernest J.; Fisch, Nathaniel J.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. RP Hay, MJ (reprint author), Princeton Univ, Dept Astrophys Sci, Princeton, NJ 08544 USA. EM hay@princeton.edu FU DOE [DE-AC02-09CH11466]; DOE NNSA SSGF [DE-FC52-08NA28752] FX This work was performed under DOE Contract No. DE-AC02-09CH11466. M.J.H. was supported by the DOE NNSA SSGF under Grant No. DE-FC52-08NA28752. NR 10 TC 3 Z9 3 U1 0 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 29 PY 2013 VL 111 IS 18 AR 188301 DI 10.1103/PhysRevLett.111.188301 PG 5 WC Physics, Multidisciplinary SC Physics GA 242XM UT WOS:000326279100022 PM 24237567 ER PT J AU Mahler, DH Rozema, LA Darabi, A Ferrie, C Blume-Kohout, R Steinberg, AM AF Mahler, D. H. Rozema, Lee A. Darabi, Ardavan Ferrie, Christopher Blume-Kohout, Robin Steinberg, A. M. TI Adaptive Quantum State Tomography Improves Accuracy Quadratically SO PHYSICAL REVIEW LETTERS LA English DT Article ID DISTANCE AB We introduce a simple protocol for adaptive quantum state tomography, which reduces the worst-case infidelity [1 - F((rho) over cap, rho)] between the estimate and the true state from O(1/root N) to O(1/N). It uses a single adaptation step and just one extra measurement setting. In a linear optical qubit experiment, we demonstrate a full order of magnitude reduction in infidelity (from 0.1% to 0.01%) for a modest number of samples (N approximate to 3 x 10(4)). C1 [Mahler, D. H.; Rozema, Lee A.; Darabi, Ardavan; Steinberg, A. M.] Univ Toronto, Ctr Quantum Informat & Quantum Control, Dept Phys, Toronto, ON M5S 1A7, Canada. [Mahler, D. H.; Rozema, Lee A.; Darabi, Ardavan; Steinberg, A. M.] Univ Toronto, Inst Opt Sci, Toronto, ON M5S 1A7, Canada. [Mahler, D. H.; Rozema, Lee A.; Darabi, Ardavan; Steinberg, A. M.] Canadian Inst Adv Res, Toronto, ON M5G 1Z8, Canada. [Ferrie, Christopher] Univ New Mexico, Ctr Quantum Informat & Control, Albuquerque, NM 87131 USA. [Blume-Kohout, Robin] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Mahler, DH (reprint author), Univ Toronto, Ctr Quantum Informat & Quantum Control, Dept Phys, 60 St George St, Toronto, ON M5S 1A7, Canada. EM dmahler@physics.utoronto.ca RI Ferrie, Christopher/C-8330-2014; Steinberg, Aephraim/C-3226-2008; OI Ferrie, Christopher/0000-0003-2736-9943 FU NSF [PHY-1212445, PHY-1005540]; LDRD program at Sandia National Laboratories; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; NSERC PDF FX D.H. M., L.A. R., A.D., and A.M.S. thank NSERC and CIFAR for support, and Alan Stummer for designing the coincidence circuit. C.F. was supported in part by NSF Grants No. PHY-1212445 and No. PHY-1005540 and an NSERC PDF. R.B.K. was supported by the LDRD program at Sandia National Laboratories, a multiprogram laboratory operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 29 TC 25 Z9 25 U1 1 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 29 PY 2013 VL 111 IS 18 AR 183601 DI 10.1103/PhysRevLett.111.183601 PG 5 WC Physics, Multidisciplinary SC Physics GA 242XM UT WOS:000326279100011 PM 24237518 ER PT J AU Rodriguez, AW Reid, MTH Intravaia, F Woolf, A Dalvit, DAR Capasso, F Johnson, SG AF Rodriguez, Alejandro W. Reid, M. T. Homer Intravaia, Francesco Woolf, Alexander Dalvit, Diego A. R. Capasso, Federico Johnson, Steven G. TI Geometry-Induced Casimir Suspension of Oblate Bodies in Fluids SO PHYSICAL REVIEW LETTERS LA English DT Article ID FORCES AB We predict that a low-permittivity oblate body (disk-shaped object) above a thin metal substrate (plate with a hole) immersed in a fluid of intermediate permittivity will experience a metastable equilibrium (restoring force) near the center of the hole. Stability is the result of a geometry-induced transition in the sign of the force, from repulsive to attractive, that occurs as the disk approaches the hole-in planar or nearly planar geometries, the same material combination yields a repulsive force at all separations, in accordance with the Dzyaloshinskii-Lifshitz-Pitaevskii condition of fluid-induced repulsion between planar bodies. We explore the stability of the system with respect to rotations and lateral translations of the disks and demonstrate interesting transitions (bifurcations) in the rotational stability of the disks as a function of their size. Finally, we consider the reciprocal situation in which the disk-plate materials are interchanged and find that in this case the system also exhibits metastability. The forces in the system are sufficiently large to be observed in experiments and should enable measurements based on the diffusion dynamics of the suspended bodies. C1 [Rodriguez, Alejandro W.] Princeton Univ, Dept Elect Engn, Princeton, NJ 08540 USA. [Reid, M. T. Homer; Johnson, Steven G.] MIT, Dept Math, Cambridge, MA 02139 USA. [Woolf, Alexander; Capasso, Federico] Harvard Univ, Sch Engn & Appl Sci, Cambridge, MA 02138 USA. [Intravaia, Francesco; Dalvit, Diego A. R.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Intravaia, Francesco] Univ Nottingham, Sch Phys & Astron, Nottingham NG7 2RD, England. RP Rodriguez, AW (reprint author), Princeton Univ, Dept Elect Engn, Princeton, NJ 08540 USA. RI Intravaia, Francesco/E-6500-2010 OI Intravaia, Francesco/0000-0001-7993-4698 FU DARPA [N66001-09-1-2070-DOD]; AFOSR Multidisciplinary Research Program of the University Research Initiative (MURI) for Complex and Robust On-chip Nanophotonics [FA9550-09-1-0704]; U.S. Army Research Office [W911NF-07-D-0004, W911NF-13-D-0001] FX This work was supported by DARPA Contract No. N66001-09-1-2070-DOD, by the AFOSR Multidisciplinary Research Program of the University Research Initiative (MURI) for Complex and Robust On-chip Nanophotonics, Grant No. FA9550-09-1-0704, and by the U.S. Army Research Office under Contracts No. W911NF-07-D-0004 and No. W911NF-13-D-0001. NR 33 TC 3 Z9 3 U1 2 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 29 PY 2013 VL 111 IS 18 AR UNSP 180402 DI 10.1103/PhysRevLett.111.180402 PG 5 WC Physics, Multidisciplinary SC Physics GA 242XM UT WOS:000326279100003 PM 24237491 ER PT J AU Gori, S Jung, S Wang, LT AF Gori, Stefania Jung, Sunghoon Wang, Lian-Tao TI Cornering electroweakinos at the LHC SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Supersymmetry Phenomenology ID MASS-DEGENERATE; LIGHTEST NEUTRALINO; SEARCH; SUPERSYMMETRY; CHARGINOS; COLLISIONS AB Squeezed supersymmetric spectra are challenging for the LHC searches based on a sizable missing energy and hard visible particles. One such scenario consists of chargino/second-lightest neutralino NLSPs and a lightest neutralino LSP with a relatively small mass gap (m(chi(NLSP)) - m(chi(LSP)) equivalent to Delta similar to (10 - 50) GeV). In this note, we explore search strategies to better probe this parameter space. We focus on the 3l + E-T(miss) channel arising from the chargino/second-lightest neutralino associated production, and we investigate the role of a relatively hard initial state radiation (ISR) jet. In addition to typical kinematic variables, such as the minimum lepton pair invariant mass, we propose an angular separation variable and two ratio variables which capitalize on the main kinematic features; leptons stay relatively soft under the boost from ISR and a sizable missing energy arises only in tight correlation with the ISR boost. With 300/fb of data at the 14 TeV LHC, we expect to probe electroweakinos up to 320 (700) GeV with Delta similar to 30 GeV and up to 220 (620) GeV with Delta similar to 20 GeV if gauginos decay via gauge bosons (light sleptons). We emphasize that the 3l channel is technically challenging for mass gaps below similar to 12 GeV. C1 [Gori, Stefania; Jung, Sunghoon; Wang, Lian-Tao] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Gori, Stefania; Jung, Sunghoon; Wang, Lian-Tao] Univ Chicago, Dept Phys, Chicago, IL 60637 USA. [Gori, Stefania] Argonne Natl Lab, HEP Div, Argonne, IL 60439 USA. [Jung, Sunghoon] Korea Inst Adv Study, Sch Phys, Seoul 130722, South Korea. [Wang, Lian-Tao] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. RP Gori, S (reprint author), Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. EM goris@uchicago.edu; nejsh21@kias.re.kr; liantaow@uchicago.edu FU DOE [de-sc0003930, DE-AC02-06CH11357, DE-FGO2-96-ER40956]; National Science Foundation [NSF PHY11-25915] FX S.G. and L.T.W would like to thank KITP for its hospitality during some part of this work has been carried out. S.J. is grateful to Chicago 2012 LHC workshop where part of this work is carried out. SJ thanks KIAS Center for Advanced Computation for providing computing resources. L. T. W. is supported by the DOE Early Career Award under grant de-sc0003930. This work is supported in part by DOE under Contract No. DE-AC02-06CH11357 (ANL), DE-FGO2-96-ER40956 (U. Chicago) and by the National Science Foundation under Grant No. NSF PHY11-25915 (KITP). NR 43 TC 27 Z9 27 U1 0 U2 2 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD OCT 29 PY 2013 IS 10 AR 191 DI 10.1007/JHEP10(2013)191 PG 20 WC Physics, Particles & Fields SC Physics GA 243DP UT WOS:000326297300001 ER PT J AU Armstrong, GSJ Colgan, J Pindzola, MS AF Armstrong, G. S. J. Colgan, J. Pindzola, M. S. TI Angular distributions for the electron-impact single ionization of sodium and magnesium SO PHYSICAL REVIEW A LA English DT Article ID COLLISIONS AB We present angular distributions for the electron-impact single ionization of sodium and magnesium at intermediate incident electron energies. The results are obtained from a full-dimensionality solution of the two-active-electron time-dependent Schrodinger equation using the time-dependent close-coupling method. We compare calculated angular distributions with existing measurements. We find good overall agreement with measurements over a range of incident electron energies in both cases. We also calculate angular distributions for ejection configurations in which no measurements are currently available. C1 [Armstrong, G. S. J.; Colgan, J.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Pindzola, M. S.] Auburn Univ, Dept Phys, Auburn, AL 36849 USA. RP Armstrong, GSJ (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. OI Colgan, James/0000-0003-1045-3858 FU National Nuclear Security Administration of the U. S. Department of Energy [DE-AC5206NA25396]; U. S. DOE; U. S. NSF FX The Los Alamos National Laboratory is operated by Los Alamos National Security, LLC for the National Nuclear Security Administration of the U. S. Department of Energy under Contract No. DE-AC5206NA25396. Computational work was carried out at Los Alamos National Laboratory through the provision of an Institutional Computing Resources award. This work was supported in part by grants from the U. S. DOE and U. S. NSF to Auburn University. We thank K. L. Nixon and A. J. Murray for useful discussions. NR 30 TC 3 Z9 4 U1 0 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1050-2947 EI 1094-1622 J9 PHYS REV A JI Phys. Rev. A PD OCT 29 PY 2013 VL 88 IS 4 AR UNSP 042713 DI 10.1103/PhysRevA.88.042713 PG 7 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA 242VH UT WOS:000326271000006 ER PT J AU Colby, R Qiao, L Zhang, KHL Shutthanandan, V Ciston, J Kabius, B Chambers, SA AF Colby, R. Qiao, L. Zhang, K. H. L. Shutthanandan, V. Ciston, J. Kabius, B. Chambers, S. A. TI Cation intermixing and electronic deviations at the insulating LaCrO3/SrTiO3(001) interface SO PHYSICAL REVIEW B LA English DT Article ID ENERGY-LOSS SPECTROSCOPY; OXIDE INTERFACES; STOICHIOMETRY; CHROMIUM; SRTIO3; GROWTH; CHARGE; TEM AB The interface between polar perovskite LaCrO3 and nonpolar SrTiO3(001) grown by molecular beam epitaxy is examined using a combination of electron microscopy, spectroscopy, and Rutherford backscattering spectrometry. The A-site cations of these ABO(3) perovskites are found to diffuse across the interface to a greater extent than the B-site cations, based on high-angle annular dark-field scanning transmission electron microscopy, energy-dispersive x-ray spectroscopy, and electron-energy-loss spectroscopy (EELS). The B-site cation valences are shown to be partially reduced near the interface by analysis of EELS near-edge structures. The location and direction of these electronic modifications do not intuitively compensate the charge imbalance imposed by uneven cation interdiffusion, and yet both the film and interface are insulating. These results highlight the importance of considering both the physical and electronic structure of such complex interfaces in determining their characteristics. C1 [Colby, R.; Shutthanandan, V.; Kabius, B.] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Qiao, L.; Zhang, K. H. L.; Chambers, S. A.] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. [Ciston, J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Natl Ctr Electron Microscopy, Berkeley, CA 94720 USA. RP Colby, R (reprint author), Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. RI Qiao, Liang/A-8165-2012; Zhang, Kelvin/F-5434-2014; Foundry, Molecular/G-9968-2014 FU US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [10122 (MBE and RBS)]; Department of Energy's Office of Biological and Environmental Research at Pacific Northwest National Laboratory; National Center for Electron Microscopy, Lawrence Berkeley National Laboratory; DOE BES [DE-AC02-05CH11231]; EMSL William Wiley Postdoctoral Fellowship program FX Thanks are extended to T. Droubay for useful discussions. This work was supported by the US Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Award No. 10122 (MBE and RBS), and the EMSL William Wiley Postdoctoral Fellowship program. The work was performed in the Environmental Molecular Sciences Laboratory, a national science user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. The authors also acknowledge support of the National Center for Electron Microscopy, Lawrence Berkeley National Laboratory, which is supported by the DOE BES under Contract No. DE-AC02-05CH11231. NR 42 TC 9 Z9 9 U1 8 U2 47 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 29 PY 2013 VL 88 IS 15 AR UNSP 155325 DI 10.1103/PhysRevB.88.155325 PG 9 WC Physics, Condensed Matter SC Physics GA 242VN UT WOS:000326272000003 ER PT J AU de la Figuera, J Novotny, Z Setvin, M Liu, TJ Mao, ZQ Chen, G N'Diaye, AT Schmid, M Diebold, U Schmid, AK Parkinson, GS AF de la Figuera, Juan Novotny, Zbynek Setvin, Martin Liu, Tijiang Mao, Zhiqiang Chen, Gong N'Diaye, Alpha T. Schmid, Michael Diebold, Ulrike Schmid, Andreas K. Parkinson, Gareth S. TI Real-space imaging of the Verwey transition at the (100) surface of magnetite SO PHYSICAL REVIEW B LA English DT Article ID ENERGY-ELECTRON MICROSCOPY; LOW-TEMPERATURE PHASE; FE3O4; POLARIZATION; PERSPECTIVE AB Effects of the Verwey transition on the (100) surface of magnetite were studied using scanning tunneling microscopy and spin polarized low-energy electron microscopy. On cooling through the transition temperature TV, the initially flat surface undergoes a rooflike distortion with a periodicity of similar to 0.5 mu m due to ferroelastic twinning within monoclinic domains of the low-temperature monoclinic structure. The monoclinic c axis orients in the surface plane, along the [001](c) directions. At the atomic scale, the charge-ordered (root 2 x root 2)R45 degrees reconstruction of the (100) surface is unperturbed by the bulk transition, and is continuous over the twin boundaries. Time resolved low-energy electron microscopy movies reveal the structural transition to be first order at the surface, indicating that the bulk transition is not an extension of the Verwey-like (root 2 x root 2)R45 degrees reconstruction. Although conceptually similar, the charge-ordered phases of the (100) surface and sub-T-V bulk of magnetite are unrelated phenomena. C1 [de la Figuera, Juan] CSIC, Inst Quim Fis Rocasolano, Madrid 28006, Spain. [Novotny, Zbynek; Setvin, Martin; Schmid, Michael; Diebold, Ulrike; Parkinson, Gareth S.] Vienna Univ Technol, Inst Appl Phys, A-1040 Vienna, Austria. [Liu, Tijiang; Mao, Zhiqiang] Tulane Univ, New Orleans, LA 70119 USA. [Chen, Gong; N'Diaye, Alpha T.; Schmid, Andreas K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP de la Figuera, J (reprint author), CSIC, Inst Quim Fis Rocasolano, Madrid 28006, Spain. EM juan.delafiguera@iqfr.csic.es RI Setvin, Martin/G-5629-2014; de la Figuera, Juan/E-7046-2010; Diebold, Ulrike/A-3681-2010; Chen, Gong/H-3074-2015; Foundry, Molecular/G-9968-2014; Setvin, Martin/G-4879-2016; OI Setvin, Martin/0000-0001-8636-921X; de la Figuera, Juan/0000-0002-7014-4777; Diebold, Ulrike/0000-0003-0319-5256; Setvin, Martin/0000-0002-1210-7740; Schmid, Michael/0000-0003-3373-9357; Parkinson, Gareth/0000-0003-2457-8977 FU Spanish Government [MAT2009-14578-C03-01, MAT2012-38045-C04-01]; Office of Basic Energy Sciences, Division of Materials and Engineering Sciences, US Department of Energy [AC0205CH11231]; Centre for Atomic-Level Catalyst Design, an Energy Frontier Research Centre; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001058]; NSF [DMR-1205469]; Austrian Science Fund [P24925-N20] FX This research was supported by the Spanish Government through Projects No. MAT2009-14578-C03-01 and No. MAT2012-38045-C04-01, by the Office of Basic Energy Sciences, Division of Materials and Engineering Sciences, US Department of Energy under Contract No. AC0205CH11231, and by the Centre for Atomic-Level Catalyst Design, an Energy Frontier Research Centre funded by the US Department of Energy, Office of Science, Office of Basic Energy Sciences under Award No. DE-SC0001058. The work at Tulane is supported by the NSF under Grant No. DMR-1205469. G.S.P. acknowledges support from the Austrian Science Fund Project No. P24925-N20. NR 40 TC 9 Z9 9 U1 2 U2 38 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 29 PY 2013 VL 88 IS 16 AR 161410 DI 10.1103/PhysRevB.88.161410 PG 5 WC Physics, Condensed Matter SC Physics GA 242VQ UT WOS:000326272400004 ER PT J AU Kadau, K Cherne, FJ Ravelo, R Germann, TC AF Kadau, Kai Cherne, Frank J. Ravelo, Ramon Germann, Timothy C. TI Shock-induced phase transformations in gallium single crystals by atomistic methods SO PHYSICAL REVIEW B LA English DT Article ID MOLECULAR-DYNAMICS SIMULATIONS; EMBEDDED-ATOM METHOD; TRANSITIONS; IMPURITIES; POTENTIALS; SURFACES; HUGONIOT; METALS; NICKEL; WAVES AB Utilizing a modified embedded atom method potential, we performed large-scale classical molecular dynamics simulations (with up to 50 million atoms) to investigate the response of Ga single crystals to shock compression along the three major orientations of the orthorhombic A11 ground state, i. e., [001], [010], and [100]. For weak shocks with particle velocity u(p) < 300 m/s, these defect-free single crystals respond elastically, but for stronger shocks, they undergo a structural phase transformation and then (for even stronger shocks) melt. For intermediate shock strengths (300 m/s < u(p) < 1.2 km/s) a split shock wave is formed, with an elastic precursor (uniaxial compression wave) leading the slower transformation wave. The transformed region consists of a mixed phase, with stripes of the product phase embedded into the uniaxially compressed parent phase, with the ratio of product to parent phase increasing with increasing shock strength, much like in martensitic phase transformations. Upon shock release from the free surface at the end of the sample, the transformation is reversed, leaving only some defects behind, which makes it difficult to experimentally investigate the structural transformation in shock-recovered samples. We investigated the structure produced by the shock and found it to be similar to the beta phase of Ga which is obtained by supercooling from the liquid state. However, the product phase shows only half the period along [100] in the calculated diffraction pattern. Further investigation showed that this is due to a different stacking sequence in this direction, namely ABCD instead of AB for the beta phase. C1 [Kadau, Kai; Germann, Timothy C.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Cherne, Frank J.] Los Alamos Natl Lab, Weapons Expt Div, Los Alamos, NM 87545 USA. [Ravelo, Ramon] Univ Texas El Paso, Dept Phys, El Paso, TX 79968 USA. RP Kadau, K (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM kadaukai@yahoo.com; cherne@lanl.gov; rravelo@utep.edu; tcg@lanl.gov OI Germann, Timothy/0000-0002-6813-238X; Cherne, Frank/0000-0002-8589-6058 FU National Nuclear Security Administration; U.S. Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396]; Advanced Simulation and Computing (ASC) program FX We would like to thank Brad Lee Holian (Los Alamos) for many interesting discussions. This work was carried out under the auspices of the National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory under contract No. DE-AC52-06NA25396, with funding by the Advanced Simulation and Computing (ASC) program. NR 42 TC 7 Z9 7 U1 4 U2 16 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD OCT 29 PY 2013 VL 88 IS 14 AR 144108 DI 10.1103/PhysRevB.88.144108 PG 10 WC Physics, Condensed Matter SC Physics GA 242VL UT WOS:000326271700002 ER PT J AU Kawano-Furukawa, H DeBeer-Schmitt, L Kikuchi, H Cameron, AS Holmes, AT Heslop, RW Forgan, EM White, JS Kihou, K Lee, CH Iyo, A Eisaki, H Saito, T Fukazawa, H Kohori, Y Gavilano, JL AF Kawano-Furukawa, H. DeBeer-Schmitt, Lisa Kikuchi, H. Cameron, A. S. Holmes, A. T. Heslop, R. W. Forgan, E. M. White, J. S. Kihou, K. Lee, C. H. Iyo, A. Eisaki, H. Saito, T. Fukazawa, H. Kohori, Y. Gavilano, J. L. TI Probing the anisotropic vortex lattice in the Fe-based superconductor KFe2As2 using small-angle neutron scattering SO PHYSICAL REVIEW B LA English DT Article AB Using small angle neutron scattering, the anisotropy of the magnetic vortex lattice (VL), in the heavily hole-doped pnictide superconductor KFe2As2, was studied. Well-ordered VL scattering patterns were measured with fields applied in directions between B parallel to c and the basal plane, rotating either towards [100] or [110]. Slightly distorted hexagonal patterns were observed when B parallel to c. However, the scattering pattern distorted more strongly as the field was rotated away from the c axis. At low field, the arrangement of vortices is affected by the anisotropy of penetration depth in the plane perpendicular to the field. By fitting the distortion with the anisotropic London model, we obtain an estimate of similar to 3.4 for the anisotropy factor gamma between the in-plane and c-axis penetration depths at the lowest temperature studied. The results further reveal VL phase transitions as a function of field direction. We discuss these transitions using the "hairy ball" theorem. C1 [Kawano-Furukawa, H.] Ochanomizu Univ, GSHS, Dept Phys, Tokyo 112, Japan. [DeBeer-Schmitt, Lisa] Oak Ridge Natl Lab, Instrument Source Div, Oak Ridge, TN USA. [Kikuchi, H.] Ochanomizu Univ, Dept Phys, Tokyo, Japan. [Cameron, A. S.; Holmes, A. T.; Heslop, R. W.; Forgan, E. M.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [White, J. S.; Gavilano, J. L.] PSI, Neutron Scattering Lab, CH-5232 Villigen, Switzerland. [White, J. S.] Ecole Polytech Fed Lausanne, Lab Quantum Magnetism, CH-1015 Lausanne, Switzerland. [Kihou, K.; Lee, C. H.; Iyo, A.; Eisaki, H.] AIST, Tsukuba, Ibaraki, Japan. [Kihou, K.; Lee, C. H.; Iyo, A.; Eisaki, H.; Fukazawa, H.; Kohori, Y.] TRIP, JST, Chiyoda, Tokyo, Japan. [Saito, T.; Fukazawa, H.; Kohori, Y.] Chiba Univ, Dept Phys, Chiba, Japan. RP Kawano-Furukawa, H (reprint author), Ochanomizu Univ, GSHS, Dept Phys, Tokyo 112, Japan. EM furukawa.hazuki@ocha.ac.jp RI White, Jonathan/G-2742-2010; DeBeer-Schmitt, Lisa/I-3313-2015; Holmes, Alexander/B-5485-2013; Kawano-Furukawa, Hazuki/M-7646-2016; Kawano-Furukawa, Hazuki/M-7695-2016 OI White, Jonathan/0000-0001-7738-0150; DeBeer-Schmitt, Lisa/0000-0001-9679-3444; Holmes, Alexander/0000-0002-3069-3069; Kawano-Furukawa, Hazuki/0000-0003-4713-3727; Kawano-Furukawa, Hazuki/0000-0003-4713-3727 FU Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy; EPSRC; MaNEP; European Commission; Ministry of Education, Culture, Sports, Science, and Technology, Japan [20102006]; Mitsubishi Foundation; US-Japan Cooperative Program on Neutron Scattering; JSPS Institutional Program for Young Researcher Overseas Visits at Ochanomizu University FX We thank M. Zolliker for invaluable assistance in setting up the dilution refrigerator at PSI, and M. Laver for discussions about the application of the HB theorem to KFe2As2. We acknowledge financial support for the part of the research conducted at ORNL's High Flux Isotope Reactor, which was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy, also the EPSRC, MaNEP and the European Commission under the 6th Framework Programme. This work was partially supported by a Grant-in-Aid for Scientific Research on Innovative Areas "Heavy Electrons" (No. 20102006) of The Ministry of Education, Culture, Sports, Science, and Technology, Japan and the Mitsubishi Foundation. The experiment using the CG2 SANS spectrometer at Oak Ridge National Laboratory was supported by the US-Japan Cooperative Program on Neutron Scattering. H. K. was supported by the JSPS Institutional Program for Young Researcher Overseas Visits at Ochanomizu University. NR 33 TC 2 Z9 2 U1 0 U2 19 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 29 PY 2013 VL 88 IS 13 AR 134524 DI 10.1103/PhysRevB.88.134524 PG 8 WC Physics, Condensed Matter SC Physics GA 242VK UT WOS:000326271500003 ER PT J AU Li, Q Cao, GX Okamoto, S Yi, JY Lin, WZ Sales, BC Yan, JQ Arita, R Kunes, J Kozhevnikov, AV Eguiluz, AG Imada, M Gai, Z Pan, MH Mandrus, DG AF Li, Qing Cao, Guixin Okamoto, Satoshi Yi, Jieyu Lin, Wenzhi Sales, Brian C. Yan, Jiaqiang Arita, Ryotaro Kunes, Jan Kozhevnikov, Anton V. Eguiluz, Adolfo G. Imada, Masatoshi Gai, Zheng Pan, Minghu Mandrus, David G. TI Atomically resolved spectroscopic study of Sr2IrO4: Experiment and theory SO SCIENTIFIC REPORTS LA English DT Article ID AUGMENTED-WAVE METHOD; TUNNELING SPECTROSCOPY; SUPERCONDUCTORS; FERROMAGNETISM; TRANSITION; DENSITY; SURFACE AB Particularly in Sr2IrO4, the interplay between spin-orbit coupling, bandwidth and on-site Coulomb repulsion stabilizes a J(eff) = 1/2 spin-orbital entangled insulating state at low temperatures. Whether this insulating phase is Mott- or Slater-type, has been under intense debate. We address this issue via spatially resolved imaging and spectroscopic studies of the Sr2IrO4 surface using scanning tunneling microscopy/spectroscopy (STM/S). STS results clearly illustrate the opening of an insulating gap (150 similar to 250 meV) below the Neel temperature (T-N), in qualitative agreement with our density-functional theory (DFT) calculations. More importantly, the temperature dependence of the gap is qualitatively consistent with our DFT 1 dynamical mean field theory (DMFT) results, both showing a continuous transition from a gapped insulating ground state to a non-gap phase as temperatures approach TN. These results indicate a significant Slater character of gap formation, thus suggesting that Sr2IrO4 is a uniquely correlated system, where Slater and Mott-Hubbard-type behaviors coexist. C1 [Li, Qing; Lin, Wenzhi; Gai, Zheng; Pan, Minghu] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Cao, Guixin; Yi, Jieyu; Yan, Jiaqiang; Mandrus, David G.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Cao, Guixin; Okamoto, Satoshi; Yi, Jieyu; Sales, Brian C.; Yan, Jiaqiang; Mandrus, David G.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Arita, Ryotaro; Imada, Masatoshi] Univ Tokyo, Dept Appl Phys, Bunkyo Ku, Tokyo 1138656, Japan. [Arita, Ryotaro; Imada, Masatoshi] JST CREST, Bunkyo Ku, Tokyo 1138656, Japan. [Kunes, Jan] Acad Sci Czech Republic, Inst Phys, Prague 16253 6, Czech Republic. [Kozhevnikov, Anton V.] ETH, Inst Theoret Phys, CH-8093 Zurich, Switzerland. [Eguiluz, Adolfo G.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Li, Qing] Soochow Univ, Inst Funct Nano & Soft Mat FUNSOM, Suzhou 215123, Jiangsu, Peoples R China. RP Pan, MH (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM panm@ornl.gov; dmandrus@utk.edu RI Okamoto, Satoshi/G-5390-2011; Kunes, Jan/B-4484-2008; Arita, Ryotaro/D-5965-2012; Gai, Zheng/B-5327-2012; Mandrus, David/H-3090-2014; Cao, Guixin/G-4452-2015 OI Okamoto, Satoshi/0000-0002-0493-7568; Kunes, Jan/0000-0001-9682-7640; Arita, Ryotaro/0000-0001-5725-072X; Gai, Zheng/0000-0002-6099-4559; Cao, Guixin/0000-0002-9252-1158 FU U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division; MEXT Japan; MEXT; Computational Materials Science Initiative (CMSI), Japan; Grant Agency of the Czech Republic [13-25251S]; ASCR; BES of the U.S. DOE; NSF [OCI-0904972] FX This research was conducted (MP, QL, ZG) at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. Research was supported (GXC, SO, WL, JYY, BCS, JQY, DGM) by the U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. RA and MI were supported by MEXT Japan and Strategic Programs for Innovative Research (SPIRE), MEXT, and the Computational Materials Science Initiative (CMSI), Japan. JK was supported by the Grant No. 13-25251S of the Grant Agency of the Czech Republic. AVK acknowledges the computational resources of the CSCS and of the NCCS and the CNMS at ORNL, which are sponsored by the respective facilities divisions of the offices of ASCR and BES of the U.S. DOE. AGE was supported by NSF Grant No. OCI-0904972. NR 48 TC 24 Z9 24 U1 5 U2 88 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD OCT 29 PY 2013 VL 3 AR 3073 DI 10.1038/srep03073 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 243QF UT WOS:000326331200001 PM 24166292 ER PT J AU Petzold, CJ Schwarz, RI AF Petzold, Christopher J. Schwarz, Richard I. TI Cells determine cell density using a small protein bound to a unique tissue-specific phospholipid SO PEERJ LA English DT Article DE Cell density signaling; Tendon morphogenesis; Bone morphogenesis; Membrane signaling; Growth plate formation AB Cell density is the critical parameter controlling tendon morphogenesis. Knowing its neighbors allows a cell to regulate correctly its proliferation and collagen production. A missing link to understanding this process is a molecular description of the sensing mechanism. Previously, this mechanism was shown in cell culture to rely on a diffusible factor (SNZR [sensor]) with an affinity for the cell layer. This led to purifying conditioned medium over 4 columns and analyzing the final column fractions for band intensity on SDS gels versus biological activity - a 16 kD band strongly correlated between assays. N-terminal sequencing - EPLAVVDL - identified a large gene (424 AA), extremely conserved between chicken and human. In this paper we probe whether this is the correct gene. Can the predicted large protein be cleaved to a smaller protein? EPLAVVDL occurs towards the C-terminus and cleavage would create a small 94 AA protein. This protein would run at similar to 10 kD, so what modifications or cofactor binding accounts for its running at 16 kD on SDS gels? This protein has no prominent hydrophobic regions, so can it be secreted? To validate its role, the chicken cDNA for this gene was tagged with myc and his and transfected into a human osteosarcoma cell line (U2OS). U2OS cells expressed the gene but not passively: differentiating into structures resembling spongy bone and expressing alkaline phosphatase, an early bone marker. Intracellularly, two bands were observed byWestern blotting: the full length protein and a smaller form (26 kD). Outside the cell, a small band (28 kD) was detected, although it was 40% larger than expected, as well asmultiple larger bands. These larger forms could be converted to the predicted smaller protein (94 AA C tags) by changing salt concentrations and ultrafiltering - releasing a cofactor to the filtrate while leaving a protein factor in the retentate. Using specific degradative enzymes and mass spectrometry, the bone cofactor was identified as a lipid containing a ceramide phosphate, a single chained glycerol lipid and a linker. Tendon uses a different cofactor made up of two fatty acid chains linked directly to the phosphate yielding a molecule about half the size. Moreover, adding the tendon factor/cofactor to osteosarcoma cells causes themto stop growing, which is opposite to its role with tendon cells. Thus, the cofactor is cell type specific both in composition and in the triggered response. Further support of its proposed role came from frozen sections from 5 week old mice where an antibody to the factor stained strongly at the growing ends of the tendon as predicted. In conclusion, the molecule needed for cell density signaling is a small protein bound to a unique, tissue-specific phospholipid yielding a membrane associated but diffusible molecule. Signal transduction is postulated to occur by an increased ordering of the plasma membrane as the concentration of this protein/lipid increases with cell density. C1 [Petzold, Christopher J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint BioEnergy Inst, Berkeley, CA 94720 USA. [Schwarz, Richard I.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. RP Schwarz, RI (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. EM rischwarz@lbl.gov FU CRADA [BG92-106]; N.I.H. [R37CA064786]; Breast Cancer Research Foundation FX This work was supported in part by a CRADA BG92-106, N.I.H. grant R37CA064786, and a grant from The Breast Cancer Research Foundation. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 32 TC 0 Z9 0 U1 1 U2 1 PU PEERJ INC PI LONDON PA 341-345 OLD ST, THIRD FLR, LONDON, EC1V 9LL, ENGLAND SN 2167-8359 J9 PEERJ JI PeerJ PD OCT 29 PY 2013 VL 1 AR e192 DI 10.7717/peerj.192 PG 35 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA V36CL UT WOS:000209190900003 PM 24244914 ER PT J AU Seagle, CT Cottrell, E Fei, YW Hummer, DR Prakapenka, VB AF Seagle, Christopher T. Cottrell, Elizabeth Fei, Yingwei Hummer, Daniel R. Prakapenka, Vitali B. TI Electrical and thermal transport properties of iron and iron-silicon alloy at high pressure SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article ID DIAMOND-ANVIL CELL; CORE CONDITIONS; EARTHS CORE; RESISTIVITY; CONDUCTIVITY; TRANSITION; NICKEL; GPA; COMPRESSION; RESISTANCE AB The efficiency of heat transfer by conduction in the Earth's core controls the dynamics of convection and limits the power available for the geodynamo. We have measured the room temperature electrical resistivity of iron and iron-silicon alloy to 60 GPa and present a new model of the resistivity at high pressures and temperatures relevant to the Earth's core. The model is compared with available shock wave data and theoretical studies. For a power law and linear temperature dependence of electrical resistivity, the calculated thermal conductivity at the core-mantle boundary is similar to 67-145W/m/K for pure Fe and similar to 41-60 W/m/K for Fe-9wt % Si. Impurities in the core have a strong effect on the transport properties of iron that could significantly impact core thermal models. The models describing the data indicate higher thermal conductivity at core pressure than previously suggested, requiring additional energy sources in the past to operate the geodynamo. C1 [Seagle, Christopher T.; Cottrell, Elizabeth] Smithsonian Inst, Natl Museum Nat Hist, Washington, DC 20560 USA. [Seagle, Christopher T.; Fei, Yingwei; Hummer, Daniel R.] Carnegie Inst Sci, Geophys Lab, Washington, DC USA. [Prakapenka, Vitali B.] Univ Chicago, Ctr Adv Radiat Sources, Chicago, IL 60637 USA. RP Seagle, CT (reprint author), Sandia Natl Labs, POB 5800,MS 1189, Albuquerque, NM 87185 USA. EM ctseagl@sandia.gov RI Fei, Yingwei/F-3709-2011 OI Fei, Yingwei/0000-0001-9955-5353 FU National Science Foundation (Earth Sciences) [EAR-0622171]; Department of Energy (Geosciences) [DE-FG02-94ER14466]; State of Illinois; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; NSF [EAR-0738654, EAR-0738741] FX Portions of this work were performed at GeoSoilEnviroCARS (Sector 13), Advanced Photon Source (APS), Argonne National Laboratory. GeoSoilEnviroCARS is supported by the National Science Foundation (Earth Sciences) under grant EAR-0622171, the Department of Energy (Geosciences) under grant DE-FG02-94ER14466, and the State of Illinois. Use of the APS was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under contract DE-AC02-06CH11357. This research was supported by NSF grant EAR-0738654 to E.C. and NSF grant EAR-0738741 to Y.F. NR 35 TC 20 Z9 21 U1 2 U2 32 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD OCT 28 PY 2013 VL 40 IS 20 BP 5377 EP 5381 DI 10.1002/2013GL057930 PG 5 WC Geosciences, Multidisciplinary SC Geology GA 301DY UT WOS:000330514200009 ER PT J AU Weijer, W Zharkov, V Nof, D Dijkstra, HA de Ruijter, WPM van Scheltinga, AT Wubs, F AF Weijer, Wilbert Zharkov, Volodymyr Nof, Doron Dijkstra, Henk A. de Ruijter, Wilhelmus P. M. van Scheltinga, Arjen Terwisscha Wubs, Fred TI Agulhas ring formation as a barotropic instability of the retroflection SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article ID ATLANTIC OVERTURNING CIRCULATION; SEPARATING MEANDERING CURRENTS; FULLY-IMPLICIT MODEL; OCEAN CIRCULATION; STEADINESS; DYNAMICS; VARIABILITY; EXCHANGE; SYSTEMS; PHYSICS AB Agulhas Leakage is an important link in the global ocean circulation, as it transfers a significant volume of relatively warm and salty water from the Indian Ocean to the Atlantic Ocean. The main route of this transfer is through the shedding of large Agulhas rings from the Agulhas retroflection. In this paper we study the dynamics of the ring formation process by analyzing the stability of the Indian/Atlantic supergyre in a reduced gravity model. We show that the ring-shedding process results from a barotropic instability of the steady circulation in the Agulhas retroflection region. The destabilizing mode appears to be linked to a Rossby basin mode of the combined South Indian/Atlantic basin, which is localized in the retroflection region by the background flow. C1 [Weijer, Wilbert] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Zharkov, Volodymyr] Ctr Ocean Atmospher Predict Studies, Tallahassee, FL USA. [Nof, Doron] Florida State Univ, Tallahassee, FL 32306 USA. [Dijkstra, Henk A.; de Ruijter, Wilhelmus P. M.] Inst Marine & Atmospher Res Utrecht, Utrecht, Netherlands. [van Scheltinga, Arjen Terwisscha] Univ Bristol, Bristol, Avon, England. [Wubs, Fred] Univ Groningen, Groningen, Netherlands. RP Weijer, W (reprint author), Los Alamos Natl Lab, CCS-2,MS B214, Los Alamos, NM 87545 USA. EM wilbert@lanl.gov RI Weijer, Wilbert/A-7909-2010; Dijkstra , Henk /H-2559-2016; de Ruijter, Wilhelmus/I-2541-2016 FU Institute for Geophysics and Planetary Physics at the Los Alamos National Laboratory; Regional and Global Climate Modeling Program of the U.S. Department of Energy Office of Science; National Nuclear Security Administration of the U.S. Department of Energy [DE-AC52-06NA25396]; COMPLEXITY project PreKurs; Netherlands Organization for Scientific Research FX This research was supported by the Institute for Geophysics and Planetary Physics at the Los Alamos National Laboratory and the Regional and Global Climate Modeling Program of the U.S. Department of Energy Office of Science. Los Alamos National Laboratory is operated by the Los Alamos National Security, LLC for the National Nuclear Security Administration of the U.S. Department of Energy under contract DE-AC52-06NA25396. H.D. acknowledges support from the COMPLEXITY project PreKurs, which was funded by the Netherlands Organization for Scientific Research. We thank Joe LaCasce and an anonymous reviewer for their constructive comments. NR 30 TC 3 Z9 3 U1 0 U2 1 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD OCT 28 PY 2013 VL 40 IS 20 BP 5435 EP 5438 DI 10.1002/2013GL057751 PG 4 WC Geosciences, Multidisciplinary SC Geology GA 301DY UT WOS:000330514200019 ER PT J AU Tang, Q Hess, PG Brown-Steiner, B Kinnison, DE AF Tang, Qi Hess, Peter G. Brown-Steiner, Benjamin Kinnison, Douglas E. TI Tropospheric ozone decrease due to the Mount Pinatubo eruption: Reduced stratospheric influx SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article ID HETEROGENEOUS CHEMISTRY; TROPICAL OZONE; MT-PINATUBO; AEROSOL; TRENDS; MODEL; MIDLATITUDES; VARIABILITY; CIRCULATION; IMPACT AB We quantify the relationship between Mount Pinatubo eruption in June 1991 and tropospheric ozone abundances. The ozone reduction in the stratosphere and troposphere following the eruption is simulated by the Whole Atmosphere Community Climate Model and is in good agreement with the ozonesonde observations. Simulated anomalies in the global stratosphere-troposphere flux of ozone following the eruption are well correlated with those in the tropospheric ozone column. Both are at their minimum in late 1992 to early 1993 (-70 Tg yr(-1) in January 1993 for the flux and -1.9 Dobson Unit in November 1992 for tropospheric ozone) and recover after 1995. Therefore, this study identifies the reduced stratosphere-to-troposphere ozone flux as an important driver of the ozone decline in the troposphere following the eruption. A large fraction (67%) of the decrease in the flux is compensated by an increase in tropospheric photochemical ozone production. While both the strength of the residual circulation and the decrease in stratospheric ozone reduce the stratospheric ozone flux, the ozone reduction is identified as the dominant cause. C1 [Tang, Qi; Hess, Peter G.; Brown-Steiner, Benjamin] Cornell Univ, Dept Biol & Environm Engn, Ithaca, NY 14853 USA. [Tang, Qi] Lawrence Livermore Natl Lab, Livermore, CA USA. [Kinnison, Douglas E.] Natl Ctr Atmospher Res, Div Atmospher Chem, Boulder, CO 80307 USA. RP Tang, Q (reprint author), Cornell Univ, Dept Biol & Environm Engn, Ithaca, NY 14853 USA. EM tang30@llnl.gov RI Tang, Qi/C-1032-2011; Hess, Peter/M-3145-2015 OI Hess, Peter/0000-0003-2439-3796 FU NSF [AGS-1042787]; National Science Foundation; U.S. Department of Energy (DOE), Office of Science, Office of Biological and Environmental Research by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Atmospheric Radiation Measurement Program of the Office of Science at the U.S. Department of Energy FX We acknowledge anonymous reviewers and the science team producing the World Ozone and Ultraviolet Radiation Data Centre (WOUDC) ozonesonde data. This work is funded by NSF grant (AGS-1042787) to Cornell University. The National Center for Atmospheric Research is operated by the University Corporation for Atmospheric Research under sponsorship of the National Science Foundation. Work at LLNL was performed under the auspices of the U.S. Department of Energy (DOE), Office of Science, Office of Biological and Environmental Research by Lawrence Livermore National Laboratory under contract DE-AC52-07NA27344 and supported by the Atmospheric Radiation Measurement Program of the Office of Science at the U.S. Department of Energy. NR 25 TC 4 Z9 4 U1 1 U2 14 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD OCT 28 PY 2013 VL 40 IS 20 BP 5553 EP 5558 DI 10.1002/2013GL056563 PG 6 WC Geosciences, Multidisciplinary SC Geology GA 301DY UT WOS:000330514200040 ER PT J AU Fu, DY Zhou, J Tongay, S Liu, K Fan, W Liu, TJK Wu, JQ AF Fu, Deyi Zhou, Jian Tongay, Sefaattin Liu, Kai Fan, Wen Liu, Tsu-Jae King Wu, Junqiao TI Mechanically modulated tunneling resistance in monolayer MoS2 SO APPLIED PHYSICS LETTERS LA English DT Article ID SURFACE AB We report on the modulation of tunneling resistance in MoS2 monolayers using a conductive atomic force microscope (AFM). The resistance between the conductive AFM probe and the bottom electrode separated by a monolayer MoS2 is reversibly reduced by up to 4 orders of magnitude, which is attributed to enhanced quantum tunneling when the monolayer is compressed by the tip force. Under the Wentzel-Kramers-Brillouim approximation, the experimental data are quantitatively explained by using the metal-insulator-metal tunneling diode model. As an ideal tunneling medium, the defect-free, nanometer-thick MoS2 monolayer can serve as the active layer for non-impacting nano-electro-mechanical switches. (C) 2013 AIP Publishing LLC. C1 [Fu, Deyi; Zhou, Jian; Tongay, Sefaattin; Liu, Kai; Fan, Wen; Wu, Junqiao] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Liu, Kai; Wu, Junqiao] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Liu, Tsu-Jae King] Univ Calif Berkeley, Dept Elect Engn & Comp Sci, Berkeley, CA 94720 USA. RP Fu, DY (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. EM wuj@berkeley.edu RI Liu, Kai/A-4754-2012; Wu, Junqiao/G-7840-2011; Fu, Deyi/C-6624-2011 OI Liu, Kai/0000-0002-0638-5189; Wu, Junqiao/0000-0002-1498-0148; Fu, Deyi/0000-0003-1365-8963 FU NSF Center for Energy Efficient Electronics Science (NSF) [ECCS-0939514] FX This work was supported by the NSF Center for Energy Efficient Electronics Science (NSF Award No. ECCS-0939514). We are grateful to Professor Eli Yablonovitch for helpful discussions. NR 18 TC 15 Z9 15 U1 1 U2 36 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD OCT 28 PY 2013 VL 103 IS 18 AR 183105 DI 10.1063/1.4827301 PG 3 WC Physics, Applied SC Physics GA 263NT UT WOS:000327816000040 ER PT J AU Liu, S Mahony, TS Bender, DA Sinclair, MB Brener, I AF Liu, Sheng Mahony, Thomas S. Bender, Daniel A. Sinclair, Michael B. Brener, Igal TI Mid-infrared time-domain spectroscopy system with carrier-envelope phase stabilization SO APPLIED PHYSICS LETTERS LA English DT Article ID FIELD-RESOLVED DETECTION; QUANTUM CASCADE LASER; REPETITION-RATE; FEMTOSECOND PULSES; GENERATION; GASE; METAMATERIAL; TRANSIENTS; THZ AB We built a mid-infrared time-domain spectroscopy (TDS) system optimized for the 8-12 mu m spectral range based on a compact ultrafast Erbium: fiber laser that enables measurements of phase-resolved optical field transients directly in the time domain with high stability and spectral brightness. We achieved long term (>10 h) stability of the TDS signal by using a carrier-envelope-phase locking technique to reduce the timing jitter caused by environmental changes. Time domain measurements of the mid-infrared beam were achieved via electro-optic sampling in a GaSe crystal, using an ultrashort (similar to 15 fs) output of the fiber laser. Here, we present a full characterization of our TDS system including the dependence of the amplitude and pulse shape of the detected infrared waveforms on the thickness of the GaSe crystals. (C) 2013 AIP Publishing LLC. C1 [Liu, Sheng; Mahony, Thomas S.; Bender, Daniel A.; Sinclair, Michael B.; Brener, Igal] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Liu, Sheng; Mahony, Thomas S.; Brener, Igal] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA. RP Liu, S (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM snliu@sandia.gov FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors thank R. Huber and A. Leitenstorfer for their help through useful discussions and initial training. This work was performed, in part, at the Center for Integrated Nanotechnologies, a U. S. Department of Energy, Office of Basic Energy Sciences user facility. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 25 TC 6 Z9 6 U1 5 U2 27 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD OCT 28 PY 2013 VL 103 IS 18 AR 181111 DI 10.1063/1.4827885 PG 5 WC Physics, Applied SC Physics GA 263NT UT WOS:000327816000076 ER PT J AU Roberts, AT Mohanta, A Everitt, HO Leach, JH Van den Broeck, D Hosalli, AM Paskova, T Bedair, SM AF Roberts, A. T. Mohanta, A. Everitt, H. O. Leach, J. H. Van den Broeck, D. Hosalli, A. M. Paskova, T. Bedair, S. M. TI Spectroscopic investigation of coupling among asymmetric InGaN/GaN multiple quantum wells grown on non-polar a-plane GaN substrates SO APPLIED PHYSICS LETTERS LA English DT Article ID LIGHT-EMITTING-DIODES; EMISSION; NITRIDE; EXCITONS AB Low defect density asymmetric multiple quantum wells (MQWs) of InGaN/GaN grown on non-polar a-plane GaN substrates were investigated using time-integrated and time-resolved photoluminescence spectroscopy. Comparison of these spectra with the predicted emission energies reveals that these QWs may be spectrally resolved at low temperatures. However, a combination of thermal activation and resonant tunneling of carriers increasingly coupled the QWs, favoring emission from the lowest energy QWs with increasing temperature in a manner analogous to MQWs composed of other non-polar semiconductor materials but unlike most InGaN MQWs grown on polar substrates and influenced by the strong polarization-dependent effects. (C) 2013 AIP Publishing LLC. C1 [Roberts, A. T.; Everitt, H. O.] US Army, Aviat & Missile Res Dev & Engn Ctr, Redstone Arsenal, AL 35898 USA. [Mohanta, A.] US Army, Aviat & Missile Res Dev & Engn Ctr, Oak Ridge Inst Sci & Educ, Res Participat Program, Redstone Arsenal, AL 35898 USA. [Everitt, H. O.] Duke Univ, Dept Phys, Durham, NC 27708 USA. [Leach, J. H.] Kyma Technol, Raleigh, NC 27617 USA. [Van den Broeck, D.; Hosalli, A. M.; Paskova, T.; Bedair, S. M.] N Carolina State Univ, Dept Elect & Comp Engn, Raleigh, NC 27695 USA. RP Paskova, T (reprint author), N Carolina State Univ, Dept Elect & Comp Engn, Raleigh, NC 27695 USA. EM tmpaskov@ncsu.edu RI Everitt, Henry/L-7118-2013 OI Everitt, Henry/0000-0002-8141-3768 FU National Science Foundation [DMR-1105842, DMR-1207075] FX This research was supported in part by appointment of A.M. to the Postgraduate Research Participation Program at the U.S. Army Aviation and Missile Research, Development and Engineering Center administered by the Oak Ridge Institute for Science and Education through an interagency agreement with the U.S. Department of Energy, as well as by National Science Foundation (Nos. DMR-1105842 and DMR-1207075). NR 26 TC 2 Z9 2 U1 1 U2 29 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD OCT 28 PY 2013 VL 103 IS 18 AR 181106 DI 10.1063/1.4827536 PG 4 WC Physics, Applied SC Physics GA 263NT UT WOS:000327816000049 ER PT J AU Luppi, E Head-Gordon, M AF Luppi, Eleonora Head-Gordon, Martin TI The role of Rydberg and continuum levels in computing high harmonic generation spectra of the hydrogen atom using time-dependent configuration interaction SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID CORRELATED MOLECULAR CALCULATIONS; ELECTRONIC OPTICAL-RESPONSE; DENSITY-FUNCTIONAL THEORY; GAUSSIAN-BASIS SETS; TD-CI SIMULATION; ULTRAFAST SCIENCE; LASER FIELDS; EOM-CCSD; ATTOSECOND; STATES AB We study the role of Rydberg bound-states and continuum levels in the field-induced electronic dynamics associated with the High-Harmonic Generation (HHG) spectroscopy of the hydrogen atom. Time-dependent configuration-interaction (TD-CI) is used with very large atomic orbital (AO) expansions (up to L = 4 with sextuple augmentation and off-center functions) to describe the bound Rydberg levels, and some continuum levels. To address the lack of ionization losses in TD-CI with finite AO basis sets, we employed a heuristic lifetime for energy levels above the ionization potential. The heuristic lifetime model is compared against the conventional atomic orbital treatment (infinite lifetimes), and a third approximation which is TD-CI using only the bound levels (continuum lifetimes go to zero). The results suggest that spectra calculated using conventional TD-CI do not converge with increasing AO basis set size, while the zero lifetime and heuristic lifetime models converge to qualitatively similar spectra, with implications for how best to apply bound state electronic structure methods to simulate HHG. The origin of HHG spectral features including the cutoff and extent of interference between peaks is uncovered by separating field-induced coupling between different types of levels (ground state, bound Rydberg levels, and continuum) in the simulated electronic dynamics. Thus the origin of deviations between the predictions of the semi-classical three step model and the full simulation can be associated with particular physical contributions, which helps to explain both the successes and the limitations of the three step model. (C) 2013 AIP Publishing LLC. C1 [Luppi, Eleonora] Univ Paris 06, Lab Chim Theor, F-75005 Paris, France. [Head-Gordon, Martin] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Head-Gordon, Martin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Luppi, E (reprint author), Univ Paris 06, Lab Chim Theor, F-75005 Paris, France. FU Department of Energy (DOE) through the USXL program at Lawrence Berkeley National Laboratory; National Science Foundation (NSF) [CHE-1048789] FX Funding for this research has been provided by the Department of Energy (DOE) through the USXL program at Lawrence Berkeley National Laboratory. We acknowledge computational resources obtained under National Science Foundation (NSF) Award No. CHE-1048789. NR 59 TC 9 Z9 9 U1 0 U2 27 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD OCT 28 PY 2013 VL 139 IS 16 AR 164121 DI 10.1063/1.4824482 PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 247RP UT WOS:000326637500024 PM 24182018 ER PT J AU Sistrunk, E Grilj, J McFarland, BK Rohlen, J Aguilar, A Guhr, M AF Sistrunk, E. Grilj, J. McFarland, B. K. Rohlen, J. Aguilar, A. Guehr, M. TI Resonant photoemission at the iron M-edge of Fe(CO)(5) SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID PHOTOELECTRON-SPECTRA; ELECTRON-SPECTROSCOPY; METAL HEXACARBONYLS; TRANSITION-METALS; CROSS-SECTIONS; PHOTON ENERGY; PHOTOIONIZATION; PENTACARBONYL; RESOLUTION; ABSORPTION AB High resolution electron kinetic energy spectra of iron pentacarbonyl (Fe(CO)(5)) are studied in the photon energy range of 40-90 eV. The relative yield of photolines associated with the Fe 3d level shows a Fano line shape at photon energies of 61 eV. The increase in signal from the 3d level is indicative of resonant photoemission involving 3p-3d transitions at the M edge of iron. The signature of this resonance is also present in photolines typically attributed to be mostly CO in character. We use the modulation depth of the Fano resonances to reinterpret the photoelectron lines in the literature. (C) 2013 AIP Publishing LLC. C1 [Sistrunk, E.; Grilj, J.; McFarland, B. K.; Guehr, M.] SLAC Natl Accelerator Lab, PULSE Inst, Menlo Pk, CA 94025 USA. [Rohlen, J.; Aguilar, A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Rohlen, J.] Univ Gothenburg, Dept Phys, SE-41296 Gothenburg, Sweden. RP Guhr, M (reprint author), SLAC Natl Accelerator Lab, PULSE Inst, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. EM mguehr@stanford.edu RI Guehr, Markus/B-7446-2015 OI Guehr, Markus/0000-0002-9111-8981 FU AMOS program within the Chemical Sciences, Geosciences, and Biosciences Division of the Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy; Office of Science Early Career Research Program through the Office of Basic Energy Sciences, U.S. Department of Energy; European Research Agency via the FP-7 PEOPLE Program (Marie Curie Action) [298210]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX The authors would like to thank the scientists and support staff at the ALS beam line 10 for their aid in setting up and performing the experiment, and Markus Koch and Kelly Gaffney for fruitful discussion. This work was supported by the AMOS program within the Chemical Sciences, Geosciences, and Biosciences Division of the Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy. M. G. acknowledges funding via the Office of Science Early Career Research Program through the Office of Basic Energy Sciences, U.S. Department of Energy. J.G. would like to acknowledge support by the European Research Agency via the FP-7 PEOPLE Program (Marie Curie Action 298210). The experiments were carried out at the Advanced Light Source, which is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 35 TC 2 Z9 2 U1 0 U2 17 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD OCT 28 PY 2013 VL 139 IS 16 AR 164318 DI 10.1063/1.4827093 PG 6 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 247RP UT WOS:000326637500046 PM 24182040 ER PT J AU Welch, PM AF Welch, P. M. TI The escape of a charged dendrimer from an oppositely charged planar surface SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID ANGLE NEUTRON-SCATTERING; RESPONSIVE CONFORMATIONAL-CHANGES; POLY(PROPYLENE IMINE) DENDRIMERS; PAMAM DENDRIMERS; MOLECULAR-DYNAMICS; POLY(AMIDOAMINE) DENDRIMERS; POLYELECTROLYTE DENDRIMERS; AQUEOUS-SOLUTIONS; STARBURST DENDRIMER; HYDRODYNAMIC RADII AB Many of the envisioned applications of dendrimers revolve around placing these molecules at and removing them from charged interfaces. Herein, we provide a prescription for the conditions needed to release a charged dendrimer from an oppositely charged flat substrate. Identifying an effective segment step length that reflects the intramolecular repulsions due to excluded volume and electrostatics, as well as the dendrimer's branching, provides the essential concept leading to an analytical prediction for the boundary between captured and free molecules. We find that this effective step length obeys trends similar to those predicted for linear chains, but is modified by the dendrimer's connectivity. Moreover, the boundary predicted for the capture of linear chains holds for dendrimers once this effective step length is employed. Monte Carlo computer simulations of coarse-grained model dendrimers escaping from charged surfaces validate these findings. The simulations consider generations 2 through 6 with a range of lengths between the branch points, as well as a range of solution ionic strengths and surface charge densities. (C) 2013 AIP Publishing LLC. C1 Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Welch, PM (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. OI Welch, Paul/0000-0001-5614-2065 FU National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396]; U.S. Department of Energy Office of Biological and Environmental Research [SCFY081004]; Los Alamos National Laboratory Directed Research and Development program FX This work was carried out under the auspices of the National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396. Financial support provided by the U.S. Department of Energy Office of Biological and Environmental Research under Proposal SCFY081004 and the Los Alamos National Laboratory Directed Research and Development program. Computing time was provided by Los Alamos National Laboratory's Institutional Computing. We thank Kim Rasmussen and Boian Alexandrov for many insightful discussions of the issues addressed herein. NR 61 TC 1 Z9 1 U1 2 U2 22 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD OCT 28 PY 2013 VL 139 IS 16 AR 164906 DI 10.1063/1.4826575 PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 247RP UT WOS:000326637500084 PM 24182078 ER PT J AU Barkov, F Romanenko, A Trenikhina, Y Grassellino, A AF Barkov, F. Romanenko, A. Trenikhina, Y. Grassellino, A. TI Precipitation of hydrides in high purity niobium after different treatments SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID HYDROGEN SYSTEM; ELECTRON-MICROSCOPE; TEMPERATURE; TANTALUM; ALLOYS AB Precipitation of lossy non-superconducting niobium hydrides represents a known problem for high purity niobium in superconducting applications. Using cryogenic optical and laser confocal scanning microscopy, we have directly observed surface precipitation and evolution of niobium hydrides in samples after different treatments used for superconducting RF cavities for particle acceleration. Precipitation is shown to occur throughout the sample volume, and the growth of hydrides is well described by the fast diffusion-controlled process in which almost all hydrogen is precipitated at T = 140 K within similar to 30 min. 120 degrees C baking and mechanical deformation are found to affect hydride precipitation through their influence on the number of nucleation and trapping centers. (C) 2013 Author(s). C1 [Barkov, F.; Romanenko, A.; Trenikhina, Y.; Grassellino, A.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Trenikhina, Y.] IIT, Dept Phys, Chicago, IL 60616 USA. RP Romanenko, A (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. EM aroman@fnal.gov FU DOE Office of Nuclear Physics; United States Department of Energy [DE-AC02-07CH11359] FX We are thankful to M. Bossert, R. Schuessler, and D. Hicks for their help with sample preparation, to S. Shishkin for the help with digital processing of the images, and to H. Padamsee for useful discussions. This work was partially funded by the DOE Office of Nuclear Physics. Fermilab is operated by Fermi Research Alliance, LLC under Contract No. DE-AC02-07CH11359 with the United States Department of Energy. NR 38 TC 8 Z9 8 U1 2 U2 9 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD OCT 28 PY 2013 VL 114 IS 16 AR 164904 DI 10.1063/1.4826901 PG 9 WC Physics, Applied SC Physics GA 247SE UT WOS:000326639200121 ER PT J AU Gao, X Nielsen, E Muller, RP Young, RW Salinger, AG Bishop, NC Lilly, MP Carroll, MS AF Gao, X. Nielsen, E. Muller, R. P. Young, R. W. Salinger, A. G. Bishop, N. C. Lilly, M. P. Carroll, M. S. TI Quantum computer aided design simulation and optimization of semiconductor quantum dots SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID FERMI-DIRAC INTEGRALS; SCHRODINGER-POISSON EQUATIONS; SELF-CONSISTENT SOLUTION; SILICON DIOXIDE; ELECTRON-STATES; DEVICES; TRANSPORT; ACCURATE; WIRES; SPIN AB We present the Quantum Computer Aided Design (QCAD) simulator that targets modeling multi-dimensional quantum devices, particularly silicon multi-quantum dots (QDs) developed for quantum bits (qubits). This finite-element simulator has three differentiating features: (i) its core contains nonlinear Poisson, effective mass Schrodinger, and Configuration Interaction solvers that have massively parallel capability for high simulation throughput and can be run individually or combined self-consistently for 1D/2D/3D quantum devices; (ii) the core solvers show superior convergence even at near-zero-Kelvin temperatures, which is critical for modeling quantum computing devices; and (iii) it interfaces directly with the full-featured optimization engine Dakota. In this work, we describe the capabilities and implementation of the QCAD simulation tool and show how it can be used to both analyze existing experimental QD devices through capacitance calculations and aid in the design of few-electron multi-QDs. In particular, we observe that computed capacitances are in rough agreement with experiment, and that quantum confinement increases capacitance when the number of electrons is fixed in a quantum dot. Coupling of QCAD with the optimizer Dakota allows for rapid identification and improvement of device layouts that are likely to exhibit few-electron quantum dot characteristics. (C) 2013 AIP Publishing LLC. C1 [Gao, X.; Nielsen, E.; Muller, R. P.; Young, R. W.; Salinger, A. G.; Bishop, N. C.; Lilly, M. P.; Carroll, M. S.] Sandia Natl Labs, Albuquerque, NM 87123 USA. RP Gao, X (reprint author), Sandia Natl Labs, 1515 Eubank SE, Albuquerque, NM 87123 USA. EM xngao@sandia.gov FU Laboratory Directed Research and Development (LDRD) program at Sandia National Laboratories; United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported by the Laboratory Directed Research and Development (LDRD) program at Sandia National Laboratories. Sandia is a Multiprogram Laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 53 TC 8 Z9 8 U1 0 U2 21 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD OCT 28 PY 2013 VL 114 IS 16 AR 164302 DI 10.1063/1.4825209 PG 19 WC Physics, Applied SC Physics GA 247SE UT WOS:000326639200080 ER PT J AU Johnson-Wilke, RL Tinberg, DS Yeager, C Qu, WG Fong, DD Fister, TT Streiffer, SK Han, YS Reaney, IM Trolier-McKinstry, S AF Johnson-Wilke, Raegan L. Tinberg, Daniel S. Yeager, C. Qu, Weiguo Fong, Dillon D. Fister, Timothy T. Streiffer, Stephen K. Han, Yisong Reaney, Ian M. Trolier-McKinstry, Susan TI Coherently strained epitaxial Pb(Zr1-xTix)O-3 thin films SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID PIEZOELECTRIC PROPERTIES; PEROVSKITES; THICKNESS; LATTICE; BATIO3; LAYER; SITU; LEAD AB Coherently strained Pb(Zr1-xTix)O-3, 0.2 <= x <= 0.35, thin films were grown by pulsed laser deposition on (001) and (111) oriented SrTiO3 substrates. A buffer layer of Pb(Zr0.6Ti0.4)O-3 was used to improve the lattice matching and induce compressive strain in Zr-rich compositions. The (001)(pc) (pc = pseudocubic) films showed an increased ferroelectric transition temperature, T-C, compared to bulk ceramics, but the transition from an untilted to a tilted ferroelectric (T-Tilt) exhibited only a modest increase in temperature. This suggests that it may be possible to enlarge the untilted ferroelectric phase field by compressive strain. Consistent with previous work on relaxed PZT films, coherently strained PZT films do not exhibit an abrupt transition from an untilted to a tilted state; rather, a region of non-zero tilt exists above T-Tilt. (111)(pc) films also showed an increased ferroelectric transition temperature with a weak strain dependence on TTilt. The compressive strain in (111)(pc) films induced a preferred domain structure with only 180 degrees domain walls, in contrast to bulk materials and relaxed films which are polydomain. (C) 2013 AIP Publishing LLC. C1 [Johnson-Wilke, Raegan L.; Tinberg, Daniel S.; Yeager, C.; Qu, Weiguo; Trolier-McKinstry, Susan] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. [Fong, Dillon D.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Fister, Timothy T.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Streiffer, Stephen K.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Han, Yisong] Univ Cambridge, Dept Mat Sci & Met, Cambridge CB3 0FS, England. [Reaney, Ian M.] Univ Sheffield, Dept Mat Sci & Engn, Sheffield S1 3JD, S Yorkshire, England. RP Johnson-Wilke, RL (reprint author), Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. OI Trolier-McKinstry, Susan/0000-0002-7267-9281 FU National Science Foundation [DMR-0602770, DMR-0820404]; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX R.L.J.-W., D. S. T., C.Y., and S.T.-M. were funded through Grants DMR-0602770 and DMR-0820404 from the National Science Foundation. D. D. F., T. T. F., and S. K. S. were supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. The use of the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. We would like to thank Dr. Jenia Karapetrova at Sector 33BM and Peter Baldo at Argonne National Laboratory for their assistance during the synchrotron diffraction experiments. NR 24 TC 4 Z9 4 U1 3 U2 37 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD OCT 28 PY 2013 VL 114 IS 16 AR 164104 DI 10.1063/1.4825215 PG 10 WC Physics, Applied SC Physics GA 247SE UT WOS:000326639200074 ER PT J AU Mahanta, NK Abramson, AR Howe, JY AF Mahanta, Nayandeep K. Abramson, Alexis R. Howe, Jane Y. TI Thermal conductivity measurements on individual vapor-grown carbon nanofibers and graphene nanoplatelets SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID ELECTRICAL-CONDUCTIVITY; PYROLYTIC-GRAPHITE; PHONON TRANSPORT; LAYER GRAPHENE; NANOTUBES; COMPOSITES; FIBERS; CONDUCTANCE; THERMOPOWER; RESISTANCE AB The thermal flash technique was utilized for measuring the thermal conductivity of vapor-grown carbon nanofibers and graphene nanoplatelets. The vapor-grown carbon nanofibers with stacked-cone morphology and heat treated to 1100 degrees C and 3000 degrees C were measured to have thermal conductivities of 1130 W/m K and 1715 W/m K, respectively. The physical dimensions of the constitutive cones determining the mean free path due to static phonon scattering were estimated to be similar to 128 nm and similar to 176 nm for the low and high heat treatment temperatures, respectively. Static scattering lengths shorter than the Umklapp scattering length indicate ballistic transport within individual cones and limit the thermal conductivities of the nanofibers. Additionally, nanoplatelets of few-layer oxygen intercalated graphene and multi-layer reduced graphene exhibited thermal conductivities of 776 W/m K and 2275 W/m K, respectively. The lower thermal conductivity of few-layer (similar to 3 layers) graphene is attributed to the presence of intercalating oxygen atoms which introduce covalent character to the interlayer interactions, acting as phonon scattering centers and hence reducing the phonon mean free path. The thermal conductivity measured for multi-layer graphene with similar to 30-45 layers lies within range of the thermal conductivities previously reported for bulk graphite. (C) 2013 AIP Publishing LLC. C1 [Mahanta, Nayandeep K.; Abramson, Alexis R.] Case Western Reserve Univ, Dept Mech & Aerosp Engn, Cleveland, OH 44106 USA. [Howe, Jane Y.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Abramson, AR (reprint author), Case Western Reserve Univ, Dept Mech & Aerosp Engn, 2123 Martin Luther King Jr Dr, Cleveland, OH 44106 USA. EM alexis.abramson@case.edu RI Howe, Jane/G-2890-2011 FU U. S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Vehicle Technologies Program; State of Ohio FX The authors would like to thank Max L. Lake and other staff at Applied Sciences, Inc. for the invaluable discussions regarding the synthesis and microstructure of the carbon nanofibers. Part of this research at the Oak Ridge National Laboratory's High Temperature Materials Laboratory was sponsored by the U. S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Vehicle Technologies Program. This work was made possible in part through financial support from the State of Ohio. The content reflects the views of the authors and does not purport to reflect the views of the State of Ohio. NR 45 TC 3 Z9 3 U1 2 U2 25 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD OCT 28 PY 2013 VL 114 IS 16 AR 163528 DI 10.1063/1.4827378 PG 8 WC Physics, Applied SC Physics GA 247SE UT WOS:000326639200040 ER PT J AU Negotia, M Hodges, MPP Bryan, MT Fry, PW Im, MY Fischer, P Allwood, DA Hayward, TJ AF Negotia, M. Hodges, M. P. P. Bryan, M. T. Fry, P. W. Im, M. -Y. Fischer, P. Allwood, D. A. Hayward, T. J. TI Linear transport of domain walls confined to propagating 1-D potential wells SO JOURNAL OF APPLIED PHYSICS LA English DT Article AB We present a method of controllably propagating domain walls (DWs) in magnetic nanowires over extended linear distances by confining them to geometrically defined energy minima. Using simple models, magnetic transmission soft x-ray microscopy and magneto-optic Kerr effect measurements, we show that the technique allows DWs to be moved at arbitrary, user-defined velocities and be positioned with micrometer precision. Our approach is expected to be of utility in applications where the precise transport and positioning of DWs take precedent over the absolute speed of propagation, for example, where the fields produced by DWs are used to trap and transport magnetized particles. (C) 2013 AIP Publishing LLC. C1 [Negotia, M.; Hodges, M. P. P.; Bryan, M. T.; Allwood, D. A.; Hayward, T. J.] Univ Sheffield, Dept Mat Sci & Engn, Sheffield S10 2TN, S Yorkshire, England. [Fry, P. W.] Univ Sheffield, Nanosci & Technol Ctr, Sheffield S10 2TN, S Yorkshire, England. [Im, M. -Y.; Fischer, P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Ctr Xray Opt, Berkeley, CA 94720 USA. RP Negotia, M (reprint author), Univ Sheffield, Dept Mat Sci & Engn, Sheffield S10 2TN, S Yorkshire, England. RI Fischer, Peter/A-3020-2010 OI Fischer, Peter/0000-0002-9824-9343 FU EPSRC [EP/J002275/1, EP/F025459/1]; Berkeley Lab's program on Magnetic Materials; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy FX This work was supported by the EPSRC (Grant Nos. EP/J002275/1 and EP/F025459/1). P. F. and M.-Y. Im acknowledge support by Berkeley Lab's program on Magnetic Materials, funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division. Portions of this work were performed as a User project at the Advanced Light Source, supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy. NR 20 TC 0 Z9 0 U1 1 U2 9 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD OCT 28 PY 2013 VL 114 IS 16 AR 163901 DI 10.1063/1.4825044 PG 6 WC Physics, Applied SC Physics GA 247SE UT WOS:000326639200056 ER PT J AU Sullivan, KT Bastea, S Kuntz, JD Gash, AE AF Sullivan, K. T. Bastea, S. Kuntz, J. D. Gash, A. E. TI A pressure-driven flow analysis of gas trapping behavior in nanocomposite thermite films SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID NANOSCALE AL/MOO3 THERMITE; REACTION PROPAGATION; COMBUSTION; AL/CUO; NANOALUMINUM; OXYGEN AB This article is in direct response to a recently published article entitled Electrophoretic deposition and mechanistic studies of nano-Al/CuO thermites (K. T. Sullivan et al., J. Appl. Phys., 112(2), 2012), in which we introduced a non-dimensional parameter as the ratio of gas production to gas escape within a thin porous thermite film. In our original analysis, we had treated the problem as Fickian diffusion of gases through the porous network. However, we believe a more physical representation of the problem is to treat this as pressure-driven flow of gases in a porous medium. We offer a new derivation of the non-dimensional parameter which calculates gas velocity using the well-known Poiseuille's Law for pressure-driven flow in a pipe. This updated analysis incorporates the porosity, gas viscosity, and pressure gradient into the equation. (C) 2013 AIP Publishing LLC. C1 [Sullivan, K. T.; Bastea, S.; Kuntz, J. D.; Gash, A. E.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RP Sullivan, KT (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344 NR 16 TC 3 Z9 3 U1 1 U2 21 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD OCT 28 PY 2013 VL 114 IS 16 AR 164907 DI 10.1063/1.4826617 PG 4 WC Physics, Applied SC Physics GA 247SE UT WOS:000326639200124 ER PT J AU Duhovic, S Oria, JV Odoh, SO Schreckenbach, G Batista, ER Diaconescu, PL AF Duhovic, Selma Oria, Jeremy V. Odoh, Samuel O. Schreckenbach, Georg Batista, Enrique R. Diaconescu, Paula L. TI Investigation of the Electronic Structure of Mono(1,1 '-Diamidoferrocene) Uranium(IV) Complexes SO ORGANOMETALLICS LA English DT Article ID TRANSITION-METAL-COMPLEXES; FERROCENE DIAMIDE LIGAND; ALKYL COMPLEXES; ABSORPTION-SPECTRA; POLYMERIZATION CATALYST; AROMATIC HETEROCYCLES; ACTINIDE COMPLEXES; REDOX CONTROL; BOND; ACTIVATION AB The electronic structure of several mono(1,1'-diamidoferrocene) uranium complexes (NNR)UX2 (NNR = fc(NR)(2), fc = 1,1'-ferrocenediyl, R = SiMe3, (SiBuMe2)-Bu-t, SiMe2Ph, X = I, CH2Ph), (NNTBS)UI(OAr) (OAr = 2,6-di-tert-butylphenoxide), and (NNTBS)U(CH2Ph)(OAr) was investigated by electrochemistry, electronic absorption and vibrational spectroscopy, and DFT calculations. Similar metrical parameters were observed for (NNTBS)U(CH2Ph)(2) and (NNDMP)U(CH2Ph)(2) (and also for the previously reported (NNTBS)UI2(THF), (NNTBS)UI2(THF), and (NNTBS)U(CH2Ph)(OAr)) that translate in similar DFT parameters (bond orders, metal charges) despite some small differences observed by electrochemistry and IR or electronic absorption spectroscopy. C1 [Duhovic, Selma; Oria, Jeremy V.; Diaconescu, Paula L.] Univ Calif Los Angeles, Dept Chem & Biochem, Los Angeles, CA 90095 USA. [Odoh, Samuel O.; Schreckenbach, Georg] Univ Manitoba, Dept Chem, Winnipeg, MB R3T 2N2, Canada. [Batista, Enrique R.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Diaconescu, PL (reprint author), Univ Calif Los Angeles, Dept Chem & Biochem, 607 Charles E Young Dr East, Los Angeles, CA 90095 USA. EM pld@chem.ucla.edu FU U.S. Department of Energy, Office of Basic Energy Sciences, Heavy Element Chemistry program [ER15984, 2012LANLE372]; LANL; Natural Sciences and Engineering Council of Canada (NSERC); Seaborg Institute for Transactinium Sciences at Los Alamos National Laboratory through a Seaborg Summer Research Fellowship FX The experimental and part of the computational work (S.D., J.V.O., P.L.D.) were supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Heavy Element Chemistry program under Grant No. ER15984 (to PLD), and the Sloan Foundation. The rest of the computational work was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Heavy Element Chemistry program under Grant No. 2012LANLE372 (to ERB). J.V.O. was supported by an LANL graduate student research fellowship during the summer of 2013. G.S. acknowledges funding from the Natural Sciences and Engineering Council of Canada (NSERC). S.O.O. has been funded by the Seaborg Institute for Transactinium Sciences at Los Alamos National Laboratory through a Seaborg Summer Research Fellowship. NR 76 TC 14 Z9 14 U1 4 U2 30 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0276-7333 EI 1520-6041 J9 ORGANOMETALLICS JI Organometallics PD OCT 28 PY 2013 VL 32 IS 20 BP 6012 EP 6021 DI 10.1021/om400521k PG 10 WC Chemistry, Inorganic & Nuclear; Chemistry, Organic SC Chemistry GA 244CY UT WOS:000326365900038 ER PT J AU Bessas, D Rushchanskii, KZ Kachlik, M Disch, S Gourdon, O Bednarcik, J Maca, K Sergueev, I Kamba, S Lezaic, M Hermann, RP AF Bessas, D. Rushchanskii, K. Z. Kachlik, M. Disch, S. Gourdon, O. Bednarcik, J. Maca, K. Sergueev, I. Kamba, S. Lezaic, M. Hermann, R. P. TI Lattice instabilities in bulk EuTiO3 SO PHYSICAL REVIEW B LA English DT Article ID X-RAY-DIFFRACTION; ATOMIC DISPLACEMENTS; MAGNETIC PROPERTIES; POWDER DIFFRACTION; SCATTERING; PEROVSKITES; RESONANCE; TITANATE; ELECTRON; CRYSTAL AB The phase purity and the lattice dynamics in bulk EuTiO3 were investigated both microscopically, using x-ray and neutron diffraction, Eu-151-Mossbauer spectroscopy, and Eu-151 nuclear inelastic scattering, and macroscopically using calorimetry, resonant ultrasound spectroscopy, and magnetometry. Furthermore, our investigations were corroborated by ab initio theoretical studies. The perovskite symmetry, Pm (3) over barm, is unstable at the M- and R-points of the Brillouin zone. The lattice instabilities are lifted when the structure relaxes in one of the symmetries: I4/mcm, Imma, R (3) over barc with relative relaxation energy around -25 meV. Intimate phase analysis confirmed phase purity of our ceramics. A prominent peak in the Eu specific density of phonon states at 11.5 meV can be modeled in all candidate symmetries. A stiffening on heating around room temperature is indicative of a phase transition similar to the one observed in SrTiO3, however, although previous studies reported the structural phase transition to the tetragonal I4/mcm phase our detailed sample purity analysis and thorough structural studies using complementary techniques did not confirm a direct phase transition. Instead, in the same temperature range, Eu delocalization is observed which might explain the lattice dynamical instabilities. C1 [Bessas, D.; Disch, S.; Sergueev, I.; Hermann, R. P.] JCNS, D-52425 Julich, Germany. [Bessas, D.; Disch, S.; Sergueev, I.; Hermann, R. P.] Forschungszentrum Julich GmbH, JARA FIT, PGI, F-38043 Grenoble, France. [Bessas, D.; Hermann, R. P.] Univ Liege, Fac Sci, B-4000 Liege, Belgium. [Rushchanskii, K. Z.; Lezaic, M.] Forschungszentrum Julich, Peter Grunberg Inst, F-38043 Grenoble, France. [Rushchanskii, K. Z.; Lezaic, M.] JARA, F-38043 Grenoble, France. [Kachlik, M.; Maca, K.] Brno Univ Technol, CEITEC, Brno 61600, Czech Republic. [Disch, S.] Inst Laue Langevin, F-38042 Grenoble, France. [Gourdon, O.] Oak Ridge Natl Lab, Neutron Scattering Sci Div, Oak Ridge, TN 37831 USA. [Gourdon, O.] Oak Ridge Natl Lab, JCNS, Oak Ridge, TN 37831 USA. [Bednarcik, J.] Deutsch Elect Synchrotron, D-22607 Hamburg, Germany. [Sergueev, I.] European Synchrotron Radiat Facil, F-38043 Grenoble, France. [Kamba, S.] Acad Sci Czech Republic, Inst Phys, Prague 18221, Czech Republic. RP Bessas, D (reprint author), European Synchrotron Radiat Facil, BP 220, F-38043 Grenoble, France. EM r.hermann@fz-juelich.de RI Lezaic, Marjana/H-8510-2013; Sergueev, Ilya/N-6591-2013; Hermann, Raphael/F-6257-2013; Kamba, Stanislav/G-5332-2014; Maca, Karel/D-7520-2012; Kachlik, Martin/D-6865-2012; Bessas, Dimitrios/I-5262-2013; Disch, Sabrina/K-7185-2013 OI Lezaic, Marjana/0000-0002-7318-9444; Sergueev, Ilya/0000-0002-7614-2238; Hermann, Raphael/0000-0002-6138-5624; Kamba, Stanislav/0000-0003-4699-869X; Kachlik, Martin/0000-0002-0619-4032; Bessas, Dimitrios/0000-0003-0240-2540; Disch, Sabrina/0000-0002-4565-189X FU Helmholtz Association of German research centers [VH NG-407, VH NG-409]; Czech Science Foundation [P204/12/1163]; MEYS [LD 11035, LD 12026 - COST MP0904]; ERDF [CEITEC - CZ.1.05/1.1.00/02.0068] FX The Helmholtz Association of German research centers is acknowledged for funding (VH NG-407 "Lattice dynamics in emerging functional materials" and VH NG-409 "Computational Nanoferronics Laboratory"). The European Synchrotron Radiation Facility, the Advanced Photon Source, the PETRAIII, and the Spallation Neutron Source are acknowledged for provision of synchrotron radiation and neutron beam time at ID22N, 6-ID-D, P02.1, POW-GEN, and NOMAD, respectively. The work in the Czech Republic has been supported by the Czech Science Foundation (Project No. P204/12/1163), MEYS (LD 11035 and LD 12026 - COST MP0904), and the ERDF (CEITEC - CZ.1.05/1.1.00/02.0068). We are grateful to Dr. D. Robinson, Dr. M. Feygenson, and Dr. J. Neuefeind for help during data acquisition and Julich Supercomputing Center for support. NR 66 TC 10 Z9 10 U1 2 U2 66 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD OCT 28 PY 2013 VL 88 IS 14 AR 144308 DI 10.1103/PhysRevB.88.144308 PG 9 WC Physics, Condensed Matter SC Physics GA 241IF UT WOS:000326159200002 ER PT J AU Korgul, A Rykaczewski, KP Grzywacz, R Sliwinska, H Batchelder, JC Bingham, C Borzov, IN Brewer, N Cartegni, L Fijalkowska, A Gross, CJ Hamilton, JH Jost, C Karny, M Krolas, W Liu, S Mazzocchi, C Madurga, M Mendez, AJ Miernik, K Miller, D Padgett, S Paulauskas, S Shapira, D Stracener, D Sieja, K Winger, JA Wolinska-Cichocka, M Zganjar, EF AF Korgul, A. Rykaczewski, K. P. Grzywacz, R. Sliwinska, H. Batchelder, J. C. Bingham, C. Borzov, I. N. Brewer, N. Cartegni, L. Fijalkowska, A. Gross, C. J. Hamilton, J. H. Jost, C. Karny, M. Krolas, W. Liu, S. Mazzocchi, C. Madurga, M. Mendez, A. J., II Miernik, K. Miller, D. Padgett, S. Paulauskas, S. Shapira, D. Stracener, D. Sieja, K. Winger, J. A. Wolinska-Cichocka, M. Zganjar, E. F. TI Experimental study of the beta-gamma and beta-n gamma decay of the neutron-rich nucleus Ga-85 SO PHYSICAL REVIEW C LA English DT Article ID SHELL-MODEL; SPECTROSCOPY AB The beta-decay properties of neutron-rich Ga-85 produced in proton-induced fission of U-238 were studied at the Holifield Radioactive Ion Beam Facility at Oak Ridge National Laboratory. Data consisted of beta - gamma and beta - gamma - gamma coincidences were collected at the Low-energy Radioactive Ion Beam Spectroscopy Station after high-resolution on-line mass separation. For the first time, the excited states in the N = 53 isotone Ge-85 were established from beta-delayed gamma decay of Ga-85. The level scheme of the N = 52 isotone Ge-84 was improved and includes now 0(+), 2(+), (2)(+), 4(+), and (0)(+) states populated in the beta-delayed-neutron-gamma decay of Ga-85. Advanced shell-model calculations were used to analyze experimental data on Ge-85 and Ge-84. C1 [Korgul, A.; Fijalkowska, A.; Karny, M.; Mazzocchi, C.; Miernik, K.] Univ Warsaw, Fac Phys, PL-00681 Warsaw, Poland. [Korgul, A.; Borzov, I. N.] Joint Inst Heavy Ion Res, Oak Ridge, TN 37831 USA. [Rykaczewski, K. P.; Grzywacz, R.; Bingham, C.; Gross, C. J.; Mendez, A. J., II; Miernik, K.; Shapira, D.; Stracener, D.; Wolinska-Cichocka, M.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Grzywacz, R.; Bingham, C.; Cartegni, L.; Madurga, M.; Miller, D.; Padgett, S.; Paulauskas, S.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Sliwinska, H.; Sieja, K.] Univ Strasbourg, IPHC, CNRS, UMR7178, F-67037 Strasbourg, France. [Batchelder, J. C.; Jost, C.; Liu, S.] Oak Ridge Associated Univ, UNIRIB, Oak Ridge, TN 37831 USA. [Borzov, I. N.] Joint Inst Nucl Res, Bogoliubov Lab Theoret Phys, Dubna 141980, Russia. [Brewer, N.; Hamilton, J. H.] Vanderbilt Univ, Dept Phys & Astron, Nashville, TN 37235 USA. [Jost, C.; Liu, S.; Wolinska-Cichocka, M.] Oak Ridge Associated Univ, ORAU, Oak Ridge, TN 37831 USA. [Krolas, W.] Polish Acad Sci, Inst Nucl Phys, PL-31342 Krakow, Poland. [Winger, J. A.] Mississippi State Univ, Dept Phys & Astron, Mississippi State, MS 39762 USA. [Wolinska-Cichocka, M.] Warsaw Univ, Heavy Ion Lab, PL-02093 Warsaw, Poland. [Zganjar, E. F.] Louisiana State Univ, Dept Phys & Astron, Baton Rouge, LA 70803 USA. RP Korgul, A (reprint author), Univ Warsaw, Fac Phys, PL-00681 Warsaw, Poland. RI Krolas, Wojciech/N-9391-2013; Miller, David/B-5372-2012 OI Miller, David/0000-0002-0426-974X FU Office of Nuclear Physics, U.S. Department of Energy; U.S. DOE [DE-AC05-00OR22725, DE-FG02-96ER41006, DE-FG02-96ER40983, DE-AC05-06OR23100, DE-FG02-96ER40978, DE-FG05-88ER40407]; National Nuclear Security Administration [DEFC03-03NA00143]; National Science Centre of the Polish Ministry of Science and Higher Education [2011/01/B/ST2/02476]; Helmholtz Alliance EMMI; IN2P3-RFBR [110291054]; U.S. Department of Energy [DE-AC05-00OR22725] FX We wish to acknowledge the Holifield Radioactive Ion Beam Facility (HRIBF) staff for their assistance with the experiments and for providing excellent quality neutron-rich radioactive beams. This research was sponsored by the Office of Nuclear Physics, U.S. Department of Energy, and supported under U.S. DOE Grants No. DE-AC05-00OR22725, No. DE-FG02-96ER41006, No. DE-FG02-96ER40983, No. DE-AC05-06OR23100, No. DE-FG02-96ER40978, and No. DE-FG05-88ER40407; National Nuclear Security Administration Grant No. DEFC03-03NA00143; National Science Centre of the Polish Ministry of Science and Higher Education Grant No. 2011/01/B/ST2/02476. I.N.B. was partially supported by Helmholtz Alliance EMMI and a grant from IN2P3-RFBR under Agreement No. 110291054. K.M.'s research was performed as a Eugene P. Wigner fellow and staff member at the Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy under Contract No. DE-AC05-00OR22725. NR 36 TC 9 Z9 9 U1 0 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD OCT 28 PY 2013 VL 88 IS 4 AR 044330 DI 10.1103/PhysRevC.88.044330 PG 6 WC Physics, Nuclear SC Physics GA 241IV UT WOS:000326161000002 ER PT J AU Marsh, JC Ma, WC Hagemann, GB Janssens, RVF Bengtsson, R Ryde, H Carpenter, MP Gurdal, G Hartley, DJ Hoffman, CR Ijaz, QA Kondev, FG Lauritsen, T Mukhopadhyay, S Riedinger, LL Yadav, RB Zhu, S AF Marsh, J. C. Ma, W. C. Hagemann, G. B. Janssens, R. V. F. Bengtsson, R. Ryde, H. Carpenter, M. P. Guerdal, G. Hartley, D. J. Hoffman, C. R. Ijaz, Q. A. Kondev, F. G. Lauritsen, T. Mukhopadhyay, S. Riedinger, L. L. Yadav, R. B. Zhu, S. TI Identification of triaxial strongly deformed bands in Hf-164 SO PHYSICAL REVIEW C LA English DT Article ID HIGH-SPIN; WOBBLING EXCITATIONS; SPECTROSCOPY; NUCLEI; MODE AB Two new rotational bands of distinct character have been identified in Hf-164. They are suggested to correspond to the long-anticipated triaxial strongly deformed (TSD) bands predicted by theoretical studies. The bands have been linked to known states, and the level spins and energies could be determined. The bands are also substantially stronger in intensity and are located at lower spins than the previously observed TSD bands in Hf-168, hereby making Hf-164 the best even-even system so far for the study of TSD structures in the A similar to 160 mass region. Cranking calculations based on the modified-oscillator model suggest that the bands are associated with four-quasiparticle configurations that involve high-j intruder (i(13/2))(2) proton orbitals. C1 [Marsh, J. C.; Ma, W. C.; Ijaz, Q. A.; Yadav, R. B.] Mississippi State Univ, Dept Phys & Astron, Mississippi State, MS 39762 USA. [Hagemann, G. B.] Niels Bohr Inst, DK-2100 Copenhagen, Denmark. [Janssens, R. V. F.; Carpenter, M. P.; Hoffman, C. R.; Lauritsen, T.; Zhu, S.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Bengtsson, R.] Lund Inst Technol, Dept Math Phys, S-22100 Lund, Sweden. [Ryde, H.] Lund Univ, Dept Nucl Phys, S-22100 Lund, Sweden. [Guerdal, G.; Kondev, F. G.] Argonne Natl Lab, Nucl Engn Div, Argonne, IL 60439 USA. [Hartley, D. J.] US Naval Acad, Dept Phys, Annapolis, MD 21402 USA. [Mukhopadhyay, S.] Bhabha Atom Res Ctr, Div Nucl Phys, Bombay 400085, Maharashtra, India. [Riedinger, L. L.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. RP Marsh, JC (reprint author), Mississippi State Univ, Dept Phys & Astron, Mississippi State, MS 39762 USA. RI Carpenter, Michael/E-4287-2015; Hoffman, Calem/H-4325-2016 OI Carpenter, Michael/0000-0002-3237-5734; Hoffman, Calem/0000-0001-7141-9827 FU U.S. Department of Energy, Office of Nuclear Physics [DE-FG02-95ER40939, DE-AC02-06CH11357]; National Science Foundation [PHY-1203100] FX The authors thank the ANL operations at Gammasphere and gratefully acknowledge the efforts of J. P. Green for the target preparation. This work was supported by the U.S. Department of Energy, Office of Nuclear Physics, under Grants No. DE-FG02-95ER40939 (MSU) and No. DE-AC02-06CH11357 (ANL) and the National Science Foundation under Grant No. PHY-1203100 (USNA). NR 30 TC 5 Z9 5 U1 0 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD OCT 28 PY 2013 VL 88 IS 4 AR 041306 DI 10.1103/PhysRevC.88.041306 PG 5 WC Physics, Nuclear SC Physics GA 241IV UT WOS:000326161000001 ER PT J AU Wiranata, A Koch, V Prakash, M Wang, XN AF Wiranata, Anton Koch, Volker Prakash, Madappa Wang, Xin Nian TI Shear viscosity of hadrons with K-matrix cross sections SO PHYSICAL REVIEW C LA English DT Article ID KINETIC GAS THEORY; HEAVY-ION COLLISIONS; PB-PB COLLISIONS; TRANSPORT-COEFFICIENTS; STATISTICAL-MECHANICS; GLUON PLASMA; TEMPERATURE; QCD AB Shear viscosity eta and entropy density s of a hadronic resonance gas are calculated using the Chapman-Enskog and virial expansion methods using the K-matrix parametrization of hadronic cross sections which preserves the unitarity of the T matrix. In the pi-K-N-eta mixture considered, a total of 57 resonances up to 2 GeV were included. Comparisons are also made to results with other hadronic cross sections such as the Breit-Wigner (BW) and, where available, experimental phase shift parameterizations. Hadronic interactions forming resonances are shown to decrease the shear viscosity and increase the entropy density leading to a substantial reduction of eta/s as the QCD phase transition temperature is approached. C1 [Wiranata, Anton; Wang, Xin Nian] Cent China Normal Univ, Inst Particle Phys, Wuhan 430079, Peoples R China. [Wiranata, Anton; Wang, Xin Nian] Cent China Normal Univ, Key Lab Quark & Lepton Phys MOE, Wuhan 430079, Peoples R China. [Wiranata, Anton; Koch, Volker; Wang, Xin Nian] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Prakash, Madappa] Ohio Univ, Dept Phys & Astron, Athens, OH 45701 USA. RP Wiranata, A (reprint author), Cent China Normal Univ, Inst Particle Phys, Wuhan 430079, Peoples R China. EM awiranata@lbl.gov; vkoch@lbl.gov; prakash@phy.ohiou.edu; xnwang@lbl.gov RI Prakash, Madappa/D-9820-2016; OI Wang, Xin-Nian/0000-0002-9734-9967 FU NSFC [11221504]; US DOE [DE-AC02-05CH11231, DE-FG02-93ER-40756] FX This work is supported by the NSFC under Grant No. 11221504, and by the US DOE under Contracts No. DE-AC02-05CH11231 and No. DE-FG02-93ER-40756. NR 67 TC 9 Z9 9 U1 0 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD OCT 28 PY 2013 VL 88 IS 4 AR 044917 DI 10.1103/PhysRevC.88.044917 PG 14 WC Physics, Nuclear SC Physics GA 241IV UT WOS:000326161000005 ER PT J AU Lees, JP Poireau, V Tisserand, V Grauges, E Palano, A Eigen, G Stugu, B Brown, DN Kerth, LT Kolomensky, YG Lee, MJ Lynch, G Koch, H Schroeder, T Hearty, C Mattison, TS McKenna, JA So, RY Khan, A Blinov, VE Buzykaev, AR Druzhinin, VP Golubev, VB Kravchenko, EA Onuchin, AP Serednyakov, SI Skovpen, YI Solodov, EP Todyshev, KY Yushkov, AN Kirkby, D Lankford, AJ Mandelkern, M Dey, B Gary, JW Long, O Vitug, GM Campagnari, C Sevilla, MF Hong, TM Kovalskyi, D Richman, JD West, CA Eisner, AM Lockman, WS Schumm, BA Seiden, A Chao, DS Cheng, CH Echenard, B Flood, KT Hitlin, DG Ongmongkolkul, P Porter, FC Andreassen, R Huard, Z Meadows, BT Pushpawela, BG Sokoloff, MD Sun, L Bloom, PC Ford, WT Gaz, A Nauenberg, U Smith, JG Wagner, SR Ayad, R Toki, WH Spaan, B Schwierz, R Bernard, D Verderi, M Playfer, S Bettoni, D Bozzi, C Calabrese, R Cibinetto, G Fioravanti, E Garzia, I Luppi, E Piemontese, L Santoro, V Baldini-Ferroli, R Calcaterra, A de Sangro, R Finocchiaro, G Martellotti, S Patteri, P Peruzzi, IM Piccolo, M Rama, M Zallo, A Contri, R Guido, E Lo Vetere, M Monge, MR Passaggio, S Patrignani, C Robutti, E Bhuyan, B Prasad, V Morii, M Adametz, A Uwer, U Lacker, HM Dauncey, PD Mallik, U Chen, C Cochran, J Meyer, WT Prell, S Gritsan, AV Arnaud, N Davier, M Derkach, D Grosdidier, G Le Diberder, F Lutz, AM Malaescu, B Roudeau, P Stocchi, A Wormser, G Lange, DJ Wright, DM Coleman, JP Fry, JR Gabathuler, E Hutchcroft, DE Payne, DJ Touramanis, C Bevan, AJ Di Lodovico, F Sacco, R Cowan, G Bougher, J Brown, DN Davis, CL Denig, AG Fritsch, M Gradl, W Griessinger, K Hafner, A Prencipe, E Schubert, KR Barlow, RJ Lafferty, GD Behn, E Cenci, R Hamilton, B Jawahery, A Roberts, DA Cowan, R Dujmic, D Sciolla, G Cheaib, R Patel, PM Robertson, SH Biassoni, P Neri, N Palombo, F Cremaldi, L Godang, R Sonnek, P Summers, DJ Simard, M Taras, P De Nardo, G Monorchio, D Onorato, G Sciacca, C Martinelli, M Raven, G Jessop, CP LoSecco, JM Honscheid, K Kass, R Brau, J Frey, R Sinev, NB Strom, D Torrence, E Feltresi, E Margoni, M Morandin, M Posocco, M Rotondo, M Simi, G Simonetto, F Stroili, R Akar, S Ben-Haim, E Bomben, M Bonneaud, GR Briand, H Calderini, G Chauveau, J Leruste, P Marchiori, G Ocariz, J Sitt, S Biasini, M Manoni, E Pacetti, S Rossi, A Angelini, C Batignani, G Bettarini, S Carpinelli, M Casarosa, G Cervelli, A Forti, F Giorgi, MA Lusiani, A Oberhof, B Paoloni, E Perez, A Rizzo, G Walsh, JJ Pegna, DL Olsen, J Smith, AJS Faccini, R Ferrarotto, F Ferroni, F Gaspero, M Gioi, LL Piredda, G Bunger, C Grunberg, O Hartmann, T Leddig, T Voss, C Waldi, R Adye, T Olaiya, EO Wilson, FF Emery, S de Monchenault, GH Vasseur, G Yeche, C Anulli, F Aston, D Bard, DJ Benitez, JF Cartaro, C Convery, MR Dorfan, J Dubois-Felsmann, GP Dunwoodie, W Ebert, M Field, RC Fulsom, BG Gabareen, AM Graham, MT Hast, C Innes, WR Kim, P Kocian, ML Leith, DWGS Lewis, P Lindemann, D Lindquist, B Luitz, S Luth, V Lynch, HL MacFarlane, DB Muller, DR Neal, H Nelson, S Perl, M Pulliam, T Ratcliff, BN Roodman, A Salnikov, AA Schindler, RH Snyder, A Su, D Sullivan, MK Va'vra, J Wagner, AP Wang, WF Wisniewski, WJ Wittgen, M Wright, DH Wulsin, HW Ziegler, V Park, W Purohit, MV White, RM Wilson, JR Randle-Conde, A Sekula, SJ Bellis, M Burchat, PR Miyashita, TS Puccio, EMT Alam, MS Ernst, JA Gorodeisky, R Guttman, N Peimer, DR Soffer, A Spanier, SM Ritchie, JL Ruland, AM Schwitters, RF Wray, BC Izen, JM Lou, XC Bianchi, F De Mori, F Filippi, A Gamba, D Zambito, S Lanceri, L Vitale, L Martinez-Vidal, F Oyanguren, A Villanueva-Perez, P Ahmed, H Albert, J Banerjee, S Bernlochner, FU Choi, HHF King, GJ Kowalewski, R Lewczuk, MJ Lueck, T Nugent, IM Roney, JM Sobie, RJ Tasneem, N Gershon, TJ Harrison, PF Latham, TE Band, HR Dasu, S Pan, Y Prepost, R Wu, SL AF Lees, J. P. Poireau, V. Tisserand, V. Grauges, E. Palano, A. Eigen, G. Stugu, B. Brown, D. N. Kerth, L. T. Kolomensky, Yu. G. Lee, M. J. Lynch, G. Koch, H. Schroeder, T. Hearty, C. Mattison, T. S. McKenna, J. A. So, R. Y. Khan, A. Blinov, V. E. Buzykaev, A. R. Druzhinin, V. P. Golubev, V. B. Kravchenko, E. A. Onuchin, A. P. Serednyakov, S. I. Skovpen, Yu. I. Solodov, E. P. Todyshev, K. Yu. Yushkov, A. N. Kirkby, D. Lankford, A. J. Mandelkern, M. Dey, B. Gary, J. W. Long, O. Vitug, G. M. Campagnari, C. Sevilla, M. Franco Hong, T. M. Kovalskyi, D. Richman, J. D. West, C. A. Eisner, A. M. Lockman, W. S. Schumm, B. A. Seiden, A. Chao, D. S. Cheng, C. H. Echenard, B. Flood, K. T. Hitlin, D. G. Ongmongkolkul, P. Porter, F. C. Andreassen, R. Huard, Z. Meadows, B. T. Pushpawela, B. G. Sokoloff, M. D. Sun, L. Bloom, P. C. Ford, W. T. Gaz, A. Nauenberg, U. Smith, J. G. Wagner, S. R. Ayad, R. Toki, W. H. Spaan, B. Schwierz, R. Bernard, D. Verderi, M. Playfer, S. Bettoni, D. Bozzi, C. Calabrese, R. Cibinetto, G. Fioravanti, E. Garzia, I. Luppi, E. Piemontese, L. Santoro, V. Baldini-Ferroli, R. Calcaterra, A. de Sangro, R. Finocchiaro, G. Martellotti, S. Patteri, P. Peruzzi, I. M. Piccolo, M. Rama, M. Zallo, A. Contri, R. Guido, E. Lo Vetere, M. Monge, M. R. Passaggio, S. Patrignani, C. Robutti, E. Bhuyan, B. Prasad, V. Morii, M. Adametz, A. Uwer, U. Lacker, H. M. Dauncey, P. D. Mallik, U. Chen, C. Cochran, J. Meyer, W. T. Prell, S. Gritsan, A. V. Arnaud, N. Davier, M. Derkach, D. Grosdidier, G. Le Diberder, F. Lutz, A. M. Malaescu, B. Roudeau, P. Stocchi, A. Wormser, G. Lange, D. J. Wright, D. M. Coleman, J. P. Fry, J. R. Gabathuler, E. Hutchcroft, D. E. Payne, D. J. Touramanis, C. Bevan, A. J. Di Lodovico, F. Sacco, R. Cowan, G. Bougher, J. Brown, D. N. Davis, C. L. Denig, A. G. Fritsch, M. Gradl, W. Griessinger, K. Hafner, A. Prencipe, E. Schubert, K. R. Barlow, R. J. Lafferty, G. D. Behn, E. Cenci, R. Hamilton, B. Jawahery, A. Roberts, D. A. Cowan, R. Dujmic, D. Sciolla, G. Cheaib, R. Patel, P. M. Robertson, S. H. Biassoni, P. Neri, N. Palombo, F. Cremaldi, L. Godang, R. Sonnek, P. Summers, D. J. Simard, M. Taras, P. De Nardo, G. Monorchio, D. Onorato, G. Sciacca, C. Martinelli, M. Raven, G. Jessop, C. P. LoSecco, J. M. Honscheid, K. Kass, R. Brau, J. Frey, R. Sinev, N. B. Strom, D. Torrence, E. Feltresi, E. Margoni, M. Morandin, M. Posocco, M. Rotondo, M. Simi, G. Simonetto, F. Stroili, R. Akar, S. Ben-Haim, E. Bomben, M. Bonneaud, G. R. Briand, H. Calderini, G. Chauveau, J. Leruste, Ph. Marchiori, G. Ocariz, J. Sitt, S. Biasini, M. Manoni, E. Pacetti, S. Rossi, A. Angelini, C. Batignani, G. Bettarini, S. Carpinelli, M. Casarosa, G. Cervelli, A. Forti, F. Giorgi, M. A. Lusiani, A. Oberhof, B. Paoloni, E. Perez, A. Rizzo, G. Walsh, J. J. Pegna, D. Lopes Olsen, J. Smith, A. J. S. Faccini, R. Ferrarotto, F. Ferroni, F. Gaspero, M. Gioi, L. Li Piredda, G. Buenger, C. Gruenberg, O. Hartmann, T. Leddig, T. Voss, C. Waldi, R. Adye, T. Olaiya, E. O. Wilson, F. F. Emery, S. de Monchenault, G. Hamel Vasseur, G. Yeche, Ch. Anulli, F. Aston, D. Bard, D. J. Benitez, J. F. Cartaro, C. Convery, M. R. Dorfan, J. Dubois-Felsmann, G. P. Dunwoodie, W. Ebert, M. Field, R. C. Fulsom, B. G. Gabareen, A. M. Graham, M. T. Hast, C. Innes, W. R. Kim, P. Kocian, M. L. Leith, D. W. G. S. Lewis, P. Lindemann, D. Lindquist, B. Luitz, S. Luth, V. Lynch, H. L. MacFarlane, D. B. Muller, D. R. Neal, H. Nelson, S. Perl, M. Pulliam, T. Ratcliff, B. N. Roodman, A. Salnikov, A. A. Schindler, R. H. Snyder, A. Su, D. Sullivan, M. K. Va'vra, J. Wagner, A. P. Wang, W. F. Wisniewski, W. J. Wittgen, M. Wright, D. H. Wulsin, H. W. Ziegler, V. Park, W. Purohit, M. V. White, R. M. Wilson, J. R. Randle-Conde, A. Sekula, S. J. Bellis, M. Burchat, P. R. Miyashita, T. S. Puccio, E. M. T. Alam, M. S. Ernst, J. A. Gorodeisky, R. Guttman, N. Peimer, D. R. Soffer, A. Spanier, S. M. Ritchie, J. L. Ruland, A. M. Schwitters, R. F. Wray, B. C. Izen, J. M. Lou, X. C. Bianchi, F. De Mori, F. Filippi, A. Gamba, D. Zambito, S. Lanceri, L. Vitale, L. Martinez-Vidal, F. Oyanguren, A. Villanueva-Perez, P. Ahmed, H. Albert, J. Banerjee, Sw. Bernlochner, F. U. Choi, H. H. F. King, G. J. Kowalewski, R. Lewczuk, M. J. Lueck, T. Nugent, I. M. Roney, J. M. Sobie, R. J. Tasneem, N. Gershon, T. J. Harrison, P. F. Latham, T. E. Band, H. R. Dasu, S. Pan, Y. Prepost, R. Wu, S. L. TI Measurement of the e(+)e(-) -> p(p)over-bar cross section in the energy range from 3.0 to 6.5 GeV SO PHYSICAL REVIEW D LA English DT Article ID LARGE MOMENTUM-TRANSFER; HADRONIC FORM-FACTORS; QUANTUM CHROMODYNAMICS; RADIATIVE-CORRECTIONS; BHABHA SCATTERING; BABAR DETECTOR; MONTE-CARLO AB The e(+)e(-) -> p (p) over bar cross section and the proton magnetic form factor have been measured in the center-of-mass energy range from 3.0 to 6.5 GeV using the initial-state radiation technique with an undetected photon. This is the first measurement of the form factor at energies higher than 4.5 GeV. The analysis is based on 469 fb-1 of integrated luminosity collected with the BABAR detector at the PEP-II collider at e(+)e(-) center-of-mass energies near 10.6 GeV. The branching fractions for the decays J/psi -> p (p) over bar and psi(2S) -> p (p) over bar have also been measured. C1 [Lees, J. P.; Poireau, V.; Tisserand, V.] Univ Savoie, CNRS, IN2P3, Lab Annecy Le Vieux Phys Particules, F-74941 Annecy Le Vieux, France. [Grauges, E.] Univ Barcelona, Fac Fis, Dept ECM, E-08028 Barcelona, Spain. [Palano, A.] Ist Nazl Fis Nucl, Sez Bari, I-70125 Bari, Italy. [Palano, A.] Univ Bari, Dipartmento Fis, I-70126 Bari, Italy. [Eigen, G.; Stugu, B.] Univ Bergen, Inst Phys, N-5007 Bergen, Norway. [Brown, D. N.; Kerth, L. T.; Kolomensky, Yu. G.; Lee, M. J.; Lynch, G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Brown, D. N.; Kerth, L. T.; Kolomensky, Yu. G.; Lee, M. J.; Lynch, G.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Koch, H.; Schroeder, T.] Ruhr Univ Bochum, Inst Expt Phys 1, D-44780 Bochum, Germany. [Hearty, C.; Mattison, T. S.; McKenna, J. A.; So, R. Y.] Univ British Columbia, Vancouver, BC V6T 1Z1, Canada. [Khan, A.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Blinov, V. E.; Buzykaev, A. R.; Druzhinin, V. P.; Golubev, V. B.; Kravchenko, E. A.; Onuchin, A. P.; Serednyakov, S. I.; Skovpen, Yu. I.; Solodov, E. P.; Todyshev, K. Yu.; Yushkov, A. N.] RAS, Budker Inst Nucl Phys, SB, Novosibirsk 630090, Russia. [Druzhinin, V. P.; Golubev, V. B.; Kravchenko, E. A.; Serednyakov, S. I.; Skovpen, Yu. I.; Solodov, E. P.; Todyshev, K. Yu.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Blinov, V. E.; Onuchin, A. P.] Novosibirsk State Tech Univ, Novosibirsk 630090, Russia. [Kirkby, D.; Lankford, A. J.; Mandelkern, M.] Univ Calif Irvine, Irvine, CA 92697 USA. [Dey, B.; Gary, J. W.; Long, O.; Vitug, G. M.] Univ Calif Riverside, Riverside, CA 92521 USA. [Campagnari, C.; Sevilla, M. Franco; Hong, T. M.; Kovalskyi, D.; Richman, J. D.; West, C. A.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Eisner, A. M.; Lockman, W. S.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Inst Particle Phys, Santa Cruz, CA 95064 USA. [Chao, D. S.; Cheng, C. H.; Echenard, B.; Flood, K. T.; Hitlin, D. G.; Ongmongkolkul, P.; Porter, F. C.] CALTECH, Pasadena, CA 91125 USA. [Andreassen, R.; Huard, Z.; Meadows, B. T.; Pushpawela, B. G.; Sokoloff, M. D.; Sun, L.] Univ Cincinnati, Cincinnati, OH 45221 USA. [Bloom, P. C.; Ford, W. T.; Gaz, A.; Nauenberg, U.; Smith, J. G.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Ayad, R.; Toki, W. H.] Colorado State Univ, Ft Collins, CO 80523 USA. [Spaan, B.] Tech Univ, Fak Phys, D-44221 Dortmund, Germany. [Schwierz, R.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Bernard, D.; Verderi, M.] Ecole Polytech, CNRS, IN2P3, Lab Leprince Ringuet, F-91128 Palaiseau, France. 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[Lusiani, A.] Scuola Normale Superiore Pisa, I-56127 Pisa, Italy. [Pegna, D. Lopes; Olsen, J.; Smith, A. J. S.] Princeton Univ, Princeton, NJ 08544 USA. [Faccini, R.; Ferrarotto, F.; Ferroni, F.; Gaspero, M.; Gioi, L. Li; Piredda, G.] Ist Nazl Fis Nucl, Sez Roma, I-00185 Rome, Italy. [Faccini, R.; Ferroni, F.; Gaspero, M.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Buenger, C.; Gruenberg, O.; Hartmann, T.; Leddig, T.; Voss, C.; Waldi, R.] Univ Rostock, D-18051 Rostock, Germany. [Adye, T.; Olaiya, E. O.; Wilson, F. F.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Emery, S.; de Monchenault, G. Hamel; Vasseur, G.; Yeche, Ch.] CEA, Ctr Saclay, SPP, Irfu, F-91191 Gif Sur Yvette, France. [Anulli, F.; Aston, D.; Bard, D. J.; Benitez, J. F.; Cartaro, C.; Convery, M. R.; Dorfan, J.; Dubois-Felsmann, G. P.; Dunwoodie, W.; Ebert, M.; Field, R. C.; Fulsom, B. G.; Gabareen, A. M.; Graham, M. T.; Hast, C.; Innes, W. R.; Kim, P.; Kocian, M. L.; Leith, D. W. G. S.; Lewis, P.; Lindemann, D.; Lindquist, B.; Luitz, S.; Luth, V.; Lynch, H. L.; MacFarlane, D. B.; Muller, D. R.; Neal, H.; Nelson, S.; Perl, M.; Pulliam, T.; Ratcliff, B. N.; Roodman, A.; Salnikov, A. A.; Schindler, R. H.; Snyder, A.; Su, D.; Sullivan, M. K.; Va'vra, J.; Wagner, A. P.; Wang, W. F.; Wisniewski, W. J.; Wittgen, M.; Wright, D. H.; Wulsin, H. W.; Ziegler, V.] SLAC, Natl Accelerator Lab, Stanford, CA 94309 USA. [Park, W.; Purohit, M. V.; White, R. M.; Wilson, J. R.] Univ S Carolina, Columbia, SC 29208 USA. [Randle-Conde, A.; Sekula, S. J.] So Methodist Univ, Dallas, TX 75275 USA. [Bellis, M.; Burchat, P. R.; Miyashita, T. S.; Puccio, E. M. T.] Stanford Univ, Stanford, CA 94305 USA. [Alam, M. S.; Ernst, J. A.] SUNY Albany, Albany, NY 12222 USA. [Gorodeisky, R.; Guttman, N.; Peimer, D. R.; Soffer, A.] Tel Aviv Univ, Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Spanier, S. M.] Univ Tennessee, Knoxville, TN 37996 USA. [Ritchie, J. L.; Ruland, A. M.; Schwitters, R. F.; Wray, B. C.] Univ Texas Austin, Austin, TX 78712 USA. [Izen, J. M.; Lou, X. C.] Univ Texas Dallas, Richardson, TX 75083 USA. [Bianchi, F.; De Mori, F.; Filippi, A.; Gamba, D.; Zambito, S.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Bianchi, F.; De Mori, F.; Gamba, D.; Zambito, S.] Univ Turin, Dipartimento Fis, I-10125 Turin, Italy. [Lanceri, L.; Vitale, L.] Ist Nazl Fis Nucl, Sez Trieste, I-34127 Trieste, Italy. [Lanceri, L.; Vitale, L.] Univ Trieste, Dipartmento Fis, I-34127 Trieste, Italy. [Martinez-Vidal, F.; Oyanguren, A.; Villanueva-Perez, P.] Univ Valencia, CSIC, IFIC, E-46071 Valencia, Spain. [Ahmed, H.; Albert, J.; Banerjee, Sw.; Bernlochner, F. U.; Choi, H. H. F.; King, G. J.; Kowalewski, R.; Lewczuk, M. J.; Lueck, T.; Nugent, I. M.; Roney, J. M.; Sobie, R. J.; Tasneem, N.] Univ Victoria, Victoria, BC V8W 3P6, Canada. [Gershon, T. J.; Harrison, P. F.; Latham, T. E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Band, H. R.; Dasu, S.; Pan, Y.; Prepost, R.; Wu, S. L.] Univ Wisconsin, Madison, WI 53706 USA. RP Lees, JP (reprint author), Univ Savoie, CNRS, IN2P3, Lab Annecy Le Vieux Phys Particules, F-74941 Annecy Le Vieux, France. RI Morandin, Mauro/A-3308-2016; Lusiani, Alberto/A-3329-2016; Di Lodovico, Francesca/L-9109-2016; Calcaterra, Alessandro/P-5260-2015; Frey, Raymond/E-2830-2016; Patrignani, Claudia/C-5223-2009; Lo Vetere, Maurizio/J-5049-2012; Lusiani, Alberto/N-2976-2015; Monge, Maria Roberta/G-9127-2012; Forti, Francesco/H-3035-2011; Oyanguren, Arantza/K-6454-2014; Luppi, Eleonora/A-4902-2015; White, Ryan/E-2979-2015; Kravchenko, Evgeniy/F-5457-2015; Calabrese, Roberto/G-4405-2015; Martinez Vidal, F*/L-7563-2014; Kolomensky, Yury/I-3510-2015 OI Morandin, Mauro/0000-0003-4708-4240; Lusiani, Alberto/0000-0002-6876-3288; Di Lodovico, Francesca/0000-0003-3952-2175; Calcaterra, Alessandro/0000-0003-2670-4826; Frey, Raymond/0000-0003-0341-2636; Patrignani, Claudia/0000-0002-5882-1747; Lo Vetere, Maurizio/0000-0002-6520-4480; Lusiani, Alberto/0000-0002-6876-3288; Monge, Maria Roberta/0000-0003-1633-3195; Forti, Francesco/0000-0001-6535-7965; Oyanguren, Arantza/0000-0002-8240-7300; Luppi, Eleonora/0000-0002-1072-5633; White, Ryan/0000-0003-3589-5900; Calabrese, Roberto/0000-0002-1354-5400; Martinez Vidal, F*/0000-0001-6841-6035; Kolomensky, Yury/0000-0001-8496-9975 FU U.S. Department of Energy; National Science Foundation; Natural Sciences and Engineering Research Council (Canada); Commissariat a l'Energie Atomique and Institut National de Physique Nucleaire et de Physique des Particules (France); Bundesministerium fur Bildung und Forschung and Deutsche Forschungsgemeinschaft (Germany); Istituto Nazionale di Fisica Nucleare (Italy); Foundation for Fundamental Research on Matter (Netherlands) FX We are grateful for the extraordinary contributions of our PEP-II colleagues in achieving the excellent luminosity and machine conditions that have made this work possible. The success of this project also relies critically on the expertise and dedication of the computing organizations that support BABAR. The collaborating institutions wish to thank SLAC for its support and the kind hospitality extended to them. This work is supported by the U.S. Department of Energy and National Science Foundation, the Natural Sciences and Engineering Research Council (Canada), the Commissariat a l'Energie Atomique and Institut National de Physique Nucleaire et de Physique des Particules (France), the Bundesministerium fur Bildung und Forschung and Deutsche Forschungsgemeinschaft (Germany), the Istituto Nazionale di Fisica Nucleare (Italy), the Foundation for Fundamental Research on Matter (Netherlands), the Research Council of Norway, the Ministry of Education and Science of the Russian Federation, Ministerio de Ciencia e Innovacion (Spain), and the Science and Technology Facilities Council (United Kingdom). Individuals have received support from the Marie-Curie IEF program (European Union) and the A. P. Sloan Foundation (U. S.). NR 27 TC 18 Z9 21 U1 0 U2 22 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD OCT 28 PY 2013 VL 88 IS 7 AR 072009 DI 10.1103/PhysRevD.88.072009 PG 12 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 241JE UT WOS:000326161900001 ER PT J AU Zheng, JX Wang, L Katsiev, K Losovyj, Y Vescovo, E Goodman, DW Dowben, PA Lu, J Mei, WN AF Zheng, Jiaxin Wang, Lu Katsiev, Khabibulakh Losovyj, Yaroslav Vescovo, Elio Goodman, D. Wayne Dowben, Peter A. Lu, Jing Mei, Wai-Ning TI Adsorption configurations of carbon monoxide on gold monolayer supported by graphene or monolayer hexagonal boron nitride: a first-principles study SO EUROPEAN PHYSICAL JOURNAL B LA English DT Article ID TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; AU NANOPARTICLES; BAND-STRUCTURE; BASIS-SET; OXIDATION; MECHANISM; SURFACES; CLUSTERS; SYSTEMS AB Using density functional theory with a semiempirical van der Waals approach proposed by Grimme, the adsorption behavior of carbon monoxide on a gold monolayer supported by graphene or monolayer hexagonal boron nitride has been investigated. Based on the changes in the Dirac cone of graphene and a Bader charge analysis, we observe that the Au(111) monolayer gains a small charge from graphene and monolayer h-BN. The adsorbed CO molecule adopts similar adsorption configurations on Au(111)/graphene and Au(111)/h-BN with Au-C distance 2.17-2.50 angstrom and Au-C-O angle of 123.9 degrees-139.6 degrees. Moreover, we found that for low CO coverages, bonding to the gold surface is surprisingly energy-favorable. Yet the CO adsorption binding energy diminishes at high coverage due to the repulsive van der Waals interactions between CO molecules. C1 [Zheng, Jiaxin; Wang, Lu; Mei, Wai-Ning] Univ Nebraska, Dept Phys, Omaha, NE 68182 USA. [Zheng, Jiaxin; Lu, Jing] Peking Univ, State Key Lab Mesoscop Phys, Beijing 100871, Peoples R China. [Zheng, Jiaxin; Lu, Jing] Peking Univ, Dept Phys, Beijing 100871, Peoples R China. [Katsiev, Khabibulakh; Goodman, D. Wayne] Texas A&M Univ, Dept Chem, College Stn, TX 77842 USA. [Losovyj, Yaroslav] Louisiana State Univ, J Bennett Johnston Sr Ctr Adv Microstruct & Devic, Baton Rouge, LA 70806 USA. [Losovyj, Yaroslav; Dowben, Peter A.] Univ Nebraska, Nebraska Ctr Mat & Nanosci, Dept Phys & Astron, Lincoln, NE 68588 USA. [Vescovo, Elio] Brookhaven Natl Lab, Natl Synchrotron Light Source, Upton, NY 11973 USA. RP Zheng, JX (reprint author), Univ Nebraska, Dept Phys, Omaha, NE 68182 USA. EM lukewl@gmail.com RI Wang, Lu/D-2528-2011; Lu, Jing/H-4248-2013 FU Nebraska Research Initiative; NSF [EPS-1010674]; DOE [DE-EE0003174]; Semiconductor Research Corporation, Division of Nanomanufacturing Sciences [2123.001]; Center for Atomic-Level Catalyst Design, an Energy Frontier Research Center; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001058]; United States Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-76CH00016]; Louisiana Board of Regents FX This work was supported by Nebraska Research Initiative, NSF EPS-1010674, DOE DE-EE0003174 and by the Semiconductor Research Corporation, Division of Nanomanufacturing Sciences, task ID 2123.001. The University of Nebraska Holland Computing Center provided the computational resources with the associated USCMS Tier-2 site at the University of Nebraska-Lincoln. Part of the experimental work was supported as part of the Center for Atomic-Level Catalyst Design, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number #DE-SC0001058. The NSLS is supported by the United States Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-76CH00016. The J. Bennett Johnston Sr. Center for Advanced Microstructures and Devices is supported by the Louisiana Board of Regents. The authors would like to acknowledge substantive discussions leading up to the paper with Nataliya Lozova, Ivan Yakovkin, and Axel Enders. NR 40 TC 1 Z9 1 U1 4 U2 50 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6028 EI 1434-6036 J9 EUR PHYS J B JI Eur. Phys. J. B PD OCT 28 PY 2013 VL 86 IS 10 AR 441 DI 10.1140/epjb/e2013-40171-7 PG 7 WC Physics, Condensed Matter SC Physics GA 244IU UT WOS:000326382200002 ER PT J AU Nomura, Y Varela, J Weinberg, SJ AF Nomura, Yasunori Varela, Jaime Weinberg, Sean J. TI Black holes or firewalls: A theory of horizons SO PHYSICAL REVIEW D LA English DT Article ID INFLATIONARY UNIVERSE; EVAPORATION; PERTURBATIONS; INFORMATION; CREATION; GRAVITY; ENTROPY AB We present a quantum theory of black hole (and other) horizons, in which the standard assumptions of complementarity are preserved without contradicting information theoretic considerations. After the scrambling time, the quantum mechanical structure of a black hole becomes that of an eternal black hole at the microscopic level. In particular, the stretched horizon degrees of freedom and the states entangled with them can be mapped into the near-horizon modes in the two exterior regions of an eternal black hole, whose mass is taken to be that of the evolving black hole at each moment. Salient features arising from this picture include (i) the number of degrees of freedom needed to describe a black hole is e(.A/2l2)P, where A is the area of the horizon; (ii) black hole states having smooth horizons, however, span only an e(A/4l2)P-dimensional subspace of the relevant e(A/2l2)P-dimensional Hilbert space; (iii) internal dynamics of the horizon is such that an infalling observer finds a smooth horizon with a probability of 1 if a state stays in this subspace. We identify the structure of local operators responsible for describing semiclassical physics in the exterior and interior spacetime regions and show that this structure avoids the arguments for firewalls-the horizon can keep being smooth throughout the evolution. We discuss the fate of infalling observers under various circumstances, especially when the observers manipulate degrees of freedom before entering the horizon, and we find that an observer can never see a firewall by making a measurement on early Hawking radiation. We also consider the presented framework from the viewpoint of an infalling reference frame and argue that Minkowski-like vacua are not unique. In particular, the number of true Minkowski vacua is infinite, although the label discriminating these vacua cannot be accessed in usual nongravitational quantum field theory. An application of the framework to de Sitter horizons is also discussed. C1 [Nomura, Yasunori] Univ Calif Berkeley, Berkeley Ctr Theoret Phys, Dept Phys, Berkeley, CA 94720 USA. Lawrence Berkeley Natl Lab, Theoret Phys Grp, Berkeley, CA 94720 USA. RP Nomura, Y (reprint author), Univ Calif Berkeley, Berkeley Ctr Theoret Phys, Dept Phys, Berkeley, CA 94720 USA. OI Nomura, Yasunori/0000-0002-1497-1479 FU Office of Science, Office of High Energy and Nuclear Physics, of the U. S. Department of Energy [DE-AC02-05CH11231]; National Science Foundation [PHY-1214644] FX We thank Juan Maldacena for useful conversations. This work was supported in part by the Director, Office of Science, Office of High Energy and Nuclear Physics, of the U. S. Department of Energy under Contract No. DE-AC02-05CH11231, and in part by the National Science Foundation under Grant No. PHY-1214644. NR 47 TC 8 Z9 8 U1 0 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD OCT 28 PY 2013 VL 88 IS 8 AR 084052 DI 10.1103/PhysRevD.88.084052 PG 13 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 241JK UT WOS:000326162700010 ER PT J AU Barai, P Nukala, PKVV Alava, MJ Zapperi, S AF Barai, Pallab Nukala, Phani K. V. V. Alava, Mikko J. Zapperi, Stefano TI Role of the sample thickness in planar crack propagation SO PHYSICAL REVIEW E LA English DT Article ID HETEROGENEOUS MATERIALS; FUSE NETWORKS; FRACTURE; DYNAMICS; STRENGTH; MODELS; MEDIA; FRONT; PAPER; BLOCK AB We study the effect of the sample thickness in planar crack front propagation in a disordered elastic medium using the random fuse model. We employ different loading conditions and we test their stability with respect to crack growth. We show that the thickness induces characteristic lengths in the stress enhancement factor in front of the crack and in the stress transfer function parallel to the crack. This is reflected by a thickness-dependent crossover scale in the crack front morphology that goes from from multiscaling to self-affine with exponents, in agreement with line depinning models and experiments. Finally, we compute the distribution of crack avalanches, which is shown to depend on the thickness and the loading mode. C1 [Barai, Pallab] Texas A&M Univ, Dept Mech Engn, College Stn, TX 77843 USA. [Nukala, Phani K. V. V.] Oak Ridge Natl Lab, Div Math & Comp Sci, Oak Ridge, TN 37831 USA. [Alava, Mikko J.] Aalto Univ, Dept Appl Phys, COMP Ctr Excellence, FIN-00076 Espoo, Finland. [Zapperi, Stefano] IENI, CNR, I-20125 Milan, Italy. [Zapperi, Stefano] ISI Fdn, I-10126 Turin, Italy. RP Barai, P (reprint author), Texas A&M Univ, Dept Mech Engn, College Stn, TX 77843 USA. RI Alava, Mikko/G-2202-2013; Zapperi, Stefano/C-9473-2009 OI Alava, Mikko/0000-0001-9249-5079; Zapperi, Stefano/0000-0001-5692-5465 FU European Research Council; Aalto University School of Science; Aalto Science Institute; Academy of Finland through the COMP Center of Excellence; Mathematical, Information, and Computational Sciences Division, Office of Advanced Scientific Computing Research, U.S. Department of Energy [DE-AC05-00OR22725]; UTBattelle, LLC FX S.Z. is supported by the European Research Council Advanced Grant 2011, SIZEFFECTS, and is grateful for the support of the visiting professor program of Aalto University School of Science and the Aalto Science Institute. M.J.A. is grateful for support from the Academy of Finland through the COMP Center of Excellence. P.K.V.V.N. acknowledges support received from the Mathematical, Information, and Computational Sciences Division, Office of Advanced Scientific Computing Research, U.S. Department of Energy, under Contract No. DE-AC05-00OR22725 with UTBattelle, LLC. NR 41 TC 3 Z9 3 U1 0 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD OCT 28 PY 2013 VL 88 IS 4 AR 042411 DI 10.1103/PhysRevE.88.042411 PG 7 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA 241JU UT WOS:000326163800008 PM 24229193 ER PT J AU Bzdak, A Skokov, V AF Bzdak, Adam Skokov, Vladimir TI Decisive Test of Color Coherence in Proton-Nucleus Collisions at the LHC SO PHYSICAL REVIEW LETTERS LA English DT Article ID HIGH-ENERGY; GLUON PRODUCTION; SCATTERING; GLASS; QCD AB Proton-nucleus collisions (p + A) at LHC energies provide a rigorous test of color glass condensate (CGC), a model proposed to describe the high energy limit of quantum chromodynamics. In the CGC the average multiplicity of charged particles at midrapidity in p + A collisions depends logarithmically on the number of participants, N-part. In contrast, the wounded nucleon model of independent nucleon-nucleon scatterings, verified at RHIC energies, predicts that multiplicity in p + A depends linearly on N-part. We argue that the dependence of mean multiplicity on N-part in p + A collisions at LHC energies can single out a model of particle production, thus offering a stringent test of the CGC and the wounded nucleon model. Based on this observation we propose a novel experimental test of color coherence in p + A collisions. C1 [Bzdak, Adam] Brookhaven Natl Lab, RIKEN, BNL Res Ctr, Upton, NY 11973 USA. [Skokov, Vladimir] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Skokov, Vladimir] Western Michigan Univ, Dept Phys, Kalamazoo, MI 49008 USA. RP Bzdak, A (reprint author), Brookhaven Natl Lab, RIKEN, BNL Res Ctr, Upton, NY 11973 USA. EM ABzdak@bnl.gov; VSkokov@quark.phy.bnl.gov OI Skokov, Vladimir/0000-0001-7619-1796 FU RIKEN-BNL Research Center; U.S. Department of Energy [DE-AC02-98CH10886] FX We thank Adrian Dumitru, Larry McLerran, and Al Mueller for valuable comments and in-depth discussions. We acknowledge Bjoern Schenke for providing us with the IP-Glasma results. Comments by Robert Pisarski, Bjoern Schenke, Paul Sorensen, and Raju Venugopalan are acknowledged. A. B. is supported through the RIKEN-BNL Research Center. V. S. is supported by the U.S. Department of Energy under Contract No. DE-AC02-98CH10886. NR 30 TC 14 Z9 14 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 28 PY 2013 VL 111 IS 18 AR 182301 DI 10.1103/PhysRevLett.111.182301 PG 5 WC Physics, Multidisciplinary SC Physics GA 241KD UT WOS:000326164800004 PM 24237511 ER PT J AU Firmo, IA Lederer, S Lupien, C Mackenzie, AP Davis, JC Kivelson, SA AF Firmo, I. A. Lederer, S. Lupien, C. Mackenzie, A. P. Davis, J. C. Kivelson, S. A. TI Evidence from tunneling spectroscopy for a quasi-one-dimensional origin of superconductivity in Sr2RuO4 SO PHYSICAL REVIEW B LA English DT Article ID SPIN-TRIPLET SUPERCONDUCTIVITY; PARTICLE INTERFERENCE; MAGNETIC-FIELDS; FERMI-SURFACE; GAP STRUCTURE; CONDUCTIVITY; FLUCTUATION; DEPENDENCE; SCATTERING; SYMMETRY AB To establish the mechanism of unconventional superconductivity in Sr2RuO4, a prerequisite is direct information concerning the momentum-space structure of the energy gaps Delta(i) (k), and in particular whether the pairing strength is stronger ("dominant") on the quasi-one-dimensional (alpha and beta) or on the quasi-two-dimensional (gamma) Fermi surfaces. We present scanning tunneling microscopy measurements of the density of states spectra in the superconducting state of Sr2RuO4 for 0.1T(c) < T < T-c and analyze them along with published thermodynamic data using a simple phenomenological model. We show that our observation of a single superconducting gap scale with maximum value 2 Delta approximate to 5T(c) along with a spectral shape indicative of line nodes is consistent, within a weak-coupling model, with magnetically mediated odd-parity superconductivity generated by dominant, near-nodal, Cooper pairing on the alpha and beta bands. C1 [Firmo, I. A.; Davis, J. C.] Cornell Univ, Dept Phys, Solid State Phys Lab, Ithaca, NY 14853 USA. [Firmo, I. A.; Davis, J. C.] Brookhaven Natl Lab, CMPMS Dept, Upton, NY 11973 USA. [Lederer, S.; Kivelson, S. A.] Stanford Univ, Dept Phys, Stanford, CA 96305 USA. [Lupien, C.] Univ Sherbrooke, Dept Phys, Sherbrooke, PQ J1K 2R1, Canada. [Lupien, C.] Univ Sherbrooke, RQMP, Sherbrooke, PQ J1K 2R1, Canada. [Mackenzie, A. P.; Davis, J. C.] Univ St Andrews, Sch Phys & Astron, St Andrews KY16 9SS, Fife, Scotland. [Mackenzie, A. P.] Max Planck Inst Chem Phys Solids, D-01187 Dresden, Germany. [Davis, J. C.] Cornell Univ, Kavli Inst Cornell Nanoscale Sci, Ithaca, NY 14853 USA. RP Firmo, IA (reprint author), Cornell Univ, Dept Phys, Solid State Phys Lab, Ithaca, NY 14853 USA. RI Mackenzie, Andrew/K-6742-2015 FU Office of Naval Research [N00014-13-1-0047]; Royal Society-Wolfson Research Merit Award; EPSRC; Fundacao para a Ciencia e a Tecnologia, Portugal [SFRH/BD/60952/2009]; [DE-AC02-76SF00515] FX We especially acknowledge and thank Y. Maeno for access to his high-quality Sr2RuO4 crystals and for many constructive comments. We thank M. Aprili, S.-B. Chung, A. Damascelli, F. Mark Fischer, E.-A. Kim, I. Mazin, S. Raghu, Jean-Philippe Reid, T. M. Rice, and A. M. Rost for helpful discussions and communications. Studies at Cornell University were supported by the Office of Naval Research under Award N00014-13-1-0047, and at Stanford under DE-AC02-76SF00515. A. P. M. acknowledges the receipt of a Royal Society-Wolfson Research Merit Award and the support of EPSRC through the Programme Grant "Topological Protection and Non-Equilibrium States in Correlated Electron Systems". I. A. F. acknowledges support from Fundacao para a Ciencia e a Tecnologia, Portugal under Fellowship No. SFRH/BD/60952/2009. C. L., I. A. F., and S. L. carried out the spectroscopic imaging STM experiments plus the data preparation and analysis; Y. M. synthesized and characterized the samples; A. P. M., J.C.D., and S. A. K. supervised the project, and wrote the paper with key contributions from S. L. and I. A. F. The manuscript reflects contribution and ideas of all authors. NR 63 TC 20 Z9 20 U1 2 U2 20 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 28 PY 2013 VL 88 IS 13 AR 134521 DI 10.1103/PhysRevB.88.134521 PG 10 WC Physics, Condensed Matter SC Physics GA 241ID UT WOS:000326159000004 ER PT J AU Lv, B Zhu, XY Lorenz, B Wei, FY Xue, YY Yin, ZP Kotliar, G Chu, CW AF Lv, B. Zhu, X. Y. Lorenz, B. Wei, F. Y. Xue, Y. Y. Yin, Z. P. Kotliar, G. Chu, C. W. TI Superconductivity in the Mn5Si3-type Zr5Sb3 system SO PHYSICAL REVIEW B LA English DT Article ID INTERSTITIAL CHEMISTRY; PHASES AB We report the discovery of superconductivity at 2.3 K in Zr5Sb3, the first superconducting member in the large compound family of the Mn5Si3-type structure. Transport, magnetic, and calorimetric measurements clearly demonstrate bulk superconductivity for Zr5Sb3 and suggest it to be a possible phonon-mediated BCS superconductor with a relatively large density of states at the Fermi level associated with the d electrons of Zr and substantially larger electron-phonon coupling compared to the Sn counterpart compound Zr5Sn3 from band structure calculations. More superconductors with even higher transition temperatures are expected to be found in this family of compounds. C1 [Lv, B.; Zhu, X. Y.; Lorenz, B.; Wei, F. Y.; Xue, Y. Y.; Chu, C. W.] Univ Houston, Dept Phys, Houston, TX 77204 USA. [Lv, B.; Zhu, X. Y.; Lorenz, B.; Wei, F. Y.; Xue, Y. Y.; Chu, C. W.] Univ Houston, Texas Ctr Superconduct, Houston, TX 77204 USA. [Yin, Z. P.; Kotliar, G.] Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08854 USA. [Chu, C. W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Lv, B (reprint author), Univ Houston, Dept Phys, Houston, TX 77204 USA. EM blv@uh.edu; cwchu@uh.edu FU US Air Force Office of Scientific Research (AFOSR) [FA9550-09-1-0656]; T.L.L. Temple Foundation; John J. and Rebecca Moores Endowment; State of Texas through the Texas Center for Superconductivity at the University of Houston; US Air Force Office of Scientific Research Multidisciplinary University Research Initiative program FX The work in Houston is supported in part by US Air Force Office of Scientific Research (AFOSR) Grant No. FA9550-09-1-0656, the T.L.L. Temple Foundation, the John J. and Rebecca Moores Endowment, and the State of Texas through the Texas Center for Superconductivity at the University of Houston. Z.P.Y. and G. K. are supported by the US Air Force Office of Scientific Research Multidisciplinary University Research Initiative program. NR 14 TC 2 Z9 2 U1 5 U2 23 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 28 PY 2013 VL 88 IS 13 AR 134520 DI 10.1103/PhysRevB.88.134520 PG 5 WC Physics, Condensed Matter SC Physics GA 241ID UT WOS:000326159000003 ER PT J AU Mayes, RL Allen, MS Kammer, DC AF Mayes, Randy L. Allen, Mathew S. Kammer, Daniel C. TI Correcting indefinite mass matrices due to substructure uncoupling SO JOURNAL OF SOUND AND VIBRATION LA English DT Article AB The transmission simulator method of experimental dynamic substructuring captures the interface forces and motions through a fixture called a transmission simulator. The transmission simulator method avoids the need to measure connection point rotations, facilitates substructuring for systems with continuous connections and enriches the modal basis of the substructure model. To use this approach, one first attaches the transmission simulator to the experimental substructure and then measures the free modes of the assembly. A finite element model of the transmission simulator is then used to subtract the transmission simulator and to couple the experimental substructure to the assembly of interest. Unfortunately, in several cases the process of subtracting the transmission simulator has caused the mass matrix for the experimental substructure to become indefinite, making the substructure model difficult or impossible to use and potentially leading to erroneous results. The authors previously developed metrics that could be used to identify which modes of the experimental model led to the indefinite mass matrix. This work presents a method that utilizes those metrics with a sensitivity analysis to adjust the transmission simulator mass matrix so that the subtraction does not produce an indefinite mass matrix. A second method is presented in which the mass matrix is made positive definite by coupling additional mass to the substructure. The methods are evaluated using both numerical and experimental test cases, showing promising results. (c) 2013 Elsevier Ltd. All rights reserved. C1 [Mayes, Randy L.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Allen, Mathew S.; Kammer, Daniel C.] Univ Wisconsin, Dept Engn Phys, Madison, WI 53706 USA. RP Allen, MS (reprint author), Univ Wisconsin, Dept Engn Phys, Madison, WI 53706 USA. EM rlmayes@sandia.gov; msallen@engr.wisc.edu; kammer@engr.wisc.edu FU Sandia National Laboratories; United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported by, and some of this work was performed at Sandia National Laboratories. Sandia is a multi-program laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL85000. NR 18 TC 4 Z9 4 U1 0 U2 5 PU ACADEMIC PRESS LTD- ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL RD, LONDON NW1 7DX, ENGLAND SN 0022-460X J9 J SOUND VIB JI J. Sound Vibr. PD OCT 28 PY 2013 VL 332 IS 22 BP 5856 EP 5866 DI 10.1016/j.jsv.2013.05.025 PG 11 WC Acoustics; Engineering, Mechanical; Mechanics SC Acoustics; Engineering; Mechanics GA 204JG UT WOS:000323361000013 ER PT J AU Lai, C Sun, X AF Lai, C. Sun, X. TI Predicting flaw-induced resonance spectrum shift with theoretical perturbation analysis SO JOURNAL OF SOUND AND VIBRATION LA English DT Article ID DAMAGE DETECTION; PLATES AB Resonance inspection is an emerging non-destructive evaluation (NDE) technique used by the automotive casting industry which uses the resonance spectra differences between the good part population and the flawed parts to identify anomalous parts. It was previously established that finite-element (FE)-based modal analysis can be used to predict the resonance spectrum for an engineering scale part with relatively good accuracy. However, FE-based simulations can be time consuming in examining the spectrum shifts induced by all possible structural flaws. This paper aims at developing a computationally efficient perturbation technique to quantify the frequency shifts induced by small structural flaws, based on the FE simulated resonance spectrum for the perfect part. A generic automotive connecting rod is used as the example part for our study. The results demonstrate that the linear perturbation theory provides a very promising way in predicting frequency changes induced by small structural flaws. As the flaw size increases, the discrepancy between the perturbation analysis and the actual FE simulation results increases due to nonlinearity, yet the perturbation analysis is still able to predict the right trend in frequency shift. Published by Elsevier Ltd. C1 [Lai, C.; Sun, X.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Sun, X (reprint author), 902 Battelle Blvd,POB 999,MSIN K7-90, Richland, WA 99352 USA. EM xin.sun@pnl.gov FU United States Department of Energy [DE-ACO5-76RL01830]; EED LDRD program at the Pacific Northwest National Laboratory FX Pacific Northwest National Laboratory is operated by Battelle for the United States Department of Energy under Contract DE-ACO5-76RL01830. This study is partially supported by the EED LDRD program at the Pacific Northwest National Laboratory. NR 19 TC 1 Z9 1 U1 1 U2 5 PU ACADEMIC PRESS LTD- ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL RD, LONDON NW1 7DX, ENGLAND SN 0022-460X J9 J SOUND VIB JI J. Sound Vibr. PD OCT 28 PY 2013 VL 332 IS 22 BP 5953 EP 5964 DI 10.1016/j.jsv.2013.05.024 PG 12 WC Acoustics; Engineering, Mechanical; Mechanics SC Acoustics; Engineering; Mechanics GA 204JG UT WOS:000323361000020 ER PT J AU Chorin, AJ Morzfeld, M AF Chorin, Alexandre J. Morzfeld, Matthias TI Conditions for successful data assimilation SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article AB [1] We show, using idealized models, that numerical data assimilation can be successful only if an effective dimension of the problem is not excessive. This effective dimension depends on the noise in the model and the data, and in physically reasonable problems, it can be moderate even when the number of variables is huge. We then analyze several data assimilation algorithms, including particle filters and variational methods. We show that well-designed particle filters can solve most of those data assimilation problems that can be solved in principle and compare the conditions under which variational methods can succeed to the conditions required of particle filters. We also discuss the limitations of our analysis. C1 [Chorin, Alexandre J.; Morzfeld, Matthias] Univ Calif Berkeley, Dept Math, Berkeley, CA 94720 USA. [Chorin, Alexandre J.; Morzfeld, Matthias] Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Morzfeld, M (reprint author), Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM mmo@math.lbl.gov FU Office of Science, Computational and Technology Research, U.S. Department of Energy [DE-AC02-05CH11231]; National Science Foundation [DMS-1217065] FX We thank P. Bickel of UC Berkeley for many interesting discussions, for making our thoughts more rigorous (where possible), and for helping us recognize the limitations of our analysis. We thank R. Miller of Oregon State University for very helpful discussions and help with the literature. We thank J. Weare for an interesting discussion. This work was supported in part by the Director, Office of Science, Computational and Technology Research, U.S. Department of Energy under contract DE-AC02-05CH11231 and by the National Science Foundation under grant DMS-1217065. NR 45 TC 7 Z9 7 U1 0 U2 5 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD OCT 27 PY 2013 VL 118 IS 20 BP 11522 EP 11533 DI 10.1002/2013JD019838 PG 12 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA V45WS UT WOS:000209847300004 ER PT J AU Davies, L Jakob, C May, P Kumar, VV Xie, S AF Davies, L. Jakob, C. May, P. Kumar, V. V. Xie, S. TI Relationships between the large-scale atmosphere and the small-scale convective state for Darwin, Australia SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article AB [1] A persistent problem for numerical weather and climate models is the representation of tropical convective precipitation which for the most part occurs on spatial and temporal scales too small and too short to be explicitly resolved. Given that model parameterizations represent this subgrid convection as a function of the large-scale atmospheric state, an understanding of the strongest relationships between the two scales is needed. This study introduces a method to create two concurrent long-term data sets that describe both the large-scale atmosphere and the characteristics of the small-scale convection. Important relationships between these two scales are then investigated. It is found that convective precipitation, through convective precipitation area, has the strongest relationship with dynamical variables such as moisture convergence and vertical velocity at midlevels. The magnitude of the fluctuations of convective strength about the mean is found to be anticorrelated with the strength of the large-scale variables, indicating a more stochastic behavior of tropical convection in weakly than strongly forced regimes, respectively. Atmospheric stability related variables are not found to be positively related to either convective precipitation area or convective precipitation intensity, which is often an assumption made in convective parameterization. On the contrary, in a more unstable atmosphere, there is lower convective precipitation. C1 [Davies, L.] Monash Univ, Sch Math, Melbourne, Vic, Australia. [Jakob, C.] Monash Univ, ARC Ctr Excellence Climate Syst Sci, Melbourne, Vic, Australia. [May, P.; Kumar, V. V.] Bur Meteorol, Ctr Australian Weather & Climate Res, Melbourne, Vic, Australia. [Xie, S.] Lawrence Livermore Natl Lab, Atmospher Sci Div, Livermore, CA USA. RP Davies, L (reprint author), Univ Melbourne, Sch Earth Sci, Melbourne, Vic 3010, Australia. EM laura.davies@unimelb.edu.au FU Office of Science (BER), U.S. Department of Energy [DE-SC0002731] FX Davies and Jakob are supported by the Office of Science (BER), U.S. Department of Energy under grant DE-SC0002731. NR 45 TC 20 Z9 20 U1 0 U2 0 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD OCT 27 PY 2013 VL 118 IS 20 BP 11534 EP 11545 DI 10.1002/jgrd.50645 PG 12 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA V45WS UT WOS:000209847300005 ER PT J AU Matsui, H Koike, M Takegawa, N Kondo, Y Takami, A Takamura, T Yoon, S Kim, SW Lim, HC Fast, JD AF Matsui, H. Koike, M. Takegawa, N. Kondo, Y. Takami, A. Takamura, T. Yoon, S. Kim, S. -W. Lim, H. -C. Fast, J. D. TI Spatial and temporal variations of new particle formation in East Asia using an NPF-explicit WRF-chem model: North-south contrast in new particle formation frequency SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article AB [1] A recently developed new particle formation (NPF)-explicit version of the Weather Research and Forecasting Chemistry (WRF-chem) model can explicitly calculate the growth and sink of nucleated clusters with 20 aerosol size bins from 1 nm to 10 mu m in diameter. In this study, the model was used to investigate spatial and temporal variations in NPF event frequency and the concentrations of aerosols (condensation nuclei, CN) and cloud condensation nuclei (CCN) within the boundary layer in East Asia in spring 2009. We found a distinct north-south contrast in the NPF frequency and mechanism in East Asia. NPF occurred mainly during limited periods over certain regions between 30 degrees and 45 degrees N (northeast China, Korea, and Japan, including regions around the active volcanoes Miyakejima and Sakurajima). In these latitudes, NPF was suppressed by high concentrations of preexisting particles under stagnant air conditions associated with high-pressure systems, although nucleation occurred more extensively during most of the simulation period. In contrast, south of 30 degrees N, nucleation and NPF were both infrequent because of low SO2 emissions and H2SO4 concentrations. The period-averaged NPF frequency at 30 degrees-45 degrees N was three times that at 20 degrees-30 degrees N. This north-south contrast in NPF frequency was validated by surface measurements in outflow regions of East Asia. The simulated period-and domain-averaged contribution of secondary particles was estimated to be 44% for CN (>10 nm) and 26% for CCN at a supersaturation of 1.0%, though the contribution was highly sensitive to the amount and size distribution of primary aerosol emissions and the rate coefficient of the nucleation parameterization. C1 [Matsui, H.; Koike, M.; Kondo, Y.] Univ Tokyo, Grad Sch Sci, Dept Earth & Planetary Sci, Tokyo, Japan. [Matsui, H.] Japan Agcy Marine Earth Sci & Technol, Res Inst Global Change, Kanagawa, Japan. [Takegawa, N.] Univ Tokyo, Res Ctr Adv Sci & Technol, Tokyo, Japan. [Takami, A.] Natl Inst Environm Studies, Tsukuba, Ibaraki, Japan. [Takamura, T.] Chiba Univ, Ctr Environm Remote Sensing, Chiba, Japan. [Yoon, S.; Kim, S. -W.] Seoul Natl Univ, Sch Earth & Environm Sci, Seoul, South Korea. [Lim, H. -C.] Korea Meteorol Adm, Climate Sci Bur, Korea Global Atmospher Watch Ctr, Taean Gun, South Korea. [Fast, J. D.] Pacific Northwest Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. RP Matsui, H (reprint author), Japan Agcy Marine Earth Sci & Technol, Res Inst Global Change, Kanazawa Ku, 3173-25 Showa Machi, Yokohama, Kanagawa 2360001, Japan. EM matsui@jamstec.go.jp RI Kondo, Yutaka/D-1459-2012 FU Ministry of Education, Culture, Sports, Science, and Technology (MEXT); Japan Science and Technology Agency (JST); Japanese Ministry of the Environment [A-0803, A-1101, B-1006]; Alliance for Global Sustainability (AGS) project, University of Tokyo; U.S. Department of Energy's (DoE) Atmospheric System Research program [DE-AC06-76RLO 1830]; School of Earth and Environmental Sciences, Seoul National University; Korea Meteorological Administration Research and Development Program [CATER 2012-3020] FX This work was supported by the Ministry of Education, Culture, Sports, Science, and Technology (MEXT), the strategic international cooperative program of the Japan Science and Technology Agency (JST), the global environment research fund of the Japanese Ministry of the Environment (A-0803, A-1101, and B-1006), and by the Alliance for Global Sustainability (AGS) project, University of Tokyo. This study was conducted as a part of the Mega-Cities: Asia Task under the framework of the International Global Atmospheric Chemistry (IGAC) project. Support for MOSAIC and WRF-Chem was provided by the U.S. Department of Energy's (DoE) Atmospheric System Research program under Contract DE-AC06-76RLO 1830 at PNNL. PNNL is operated for the U.S. DoE by the Battelle Memorial Institute. For a part of the simulations, we used the HA8000 computer system operated by the Supercomputing Division, Information Technology Center, University of Tokyo. S.-C. Yoon and S.-W. Kim were supported by the BK21 program of the School of Earth and Environmental Sciences, Seoul National University, and by the Korea Meteorological Administration Research and Development Program under Grant CATER 2012-3020. NR 118 TC 14 Z9 14 U1 4 U2 31 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD OCT 27 PY 2013 VL 118 IS 20 BP 11647 EP 11663 DI 10.1002/jgrd.50821 PG 17 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA V45WS UT WOS:000209847300014 ER PT J AU Song, C Gyawali, M Zaveri, RA Shilling, JE Arnott, WP AF Song, Chen Gyawali, Madhu Zaveri, Rahul A. Shilling, John E. Arnott, W. Patrick TI Light absorption by secondary organic aerosol from alpha-pinene: Effects of oxidants, seed aerosol acidity, and relative humidity SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article AB [1] It is well known that light absorption from dust and black carbon aerosols has a warming effect on climate while light scattering from sulfate, nitrate, and sea salt aerosols has a cooling effect. However, there are large uncertainties associated with light absorption and scattering by different types of organic aerosols, especially in the near-UV and UV spectral regions. In this paper, we present the results from a systematic laboratory study focused on measuring light absorption by secondary organic aerosols (SOAs) generated from dark alpha-pinene + O-3 and alpha-pinene + NOx + O-3 systems in the presence of neutral and acidic sulfate seed aerosols. Light absorption was monitored using photoacoustic spectrometers at four different wavelengths: 355, 405, 532, and 870 nm. Significant light absorption at 355 and 405 nm was observed for the SOA formed from alpha-pinene + O-3 + NO3 system only in the presence of highly acidic sulfate seed aerosols under dry conditions. In contrast, no absorption was observed when the relative humidity was elevated to greater than 27% or in the presence of neutral sulfate seed aerosols. Organic nitrates in the SOA formed in the presence of neutral sulfate seed aerosols were found to be nonabsorbing, while the light-absorbing compounds are speculated to be aldol condensation oligomers with nitroxy organosulfate groups that are formed in highly acidic sulfate aerosols. Overall, these results suggest that dark alpha-pinene + O-3 and alpha-pinene + NOx + O-3 systems do not form light-absorbing SOA under typical atmospheric conditions. C1 [Song, Chen; Zaveri, Rahul A.; Shilling, John E.] Pacific Northwest Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. [Gyawali, Madhu; Arnott, W. Patrick] Univ Nevada Reno, Dept Phys, Nevada Syst Higher Educ, Reno, NV USA. RP Song, C (reprint author), RJ Reynolds Tobacco Co, 401 N Main St, Winston Salem, NC 27101 USA. EM songc@rjrt.com; rahul.zaveri@pnnl.gov OI Zaveri, Rahul/0000-0001-9874-8807 FU U.S. Department of Energy's (DOE) Atmospheric System Research (ASR) program; Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility - DOE's Office of Biological and Environmental Research; U.S. Department of Energy [DE-AC06-76RLO1830] FX We thank Alexander Laskin (PNNL) for thoughtful suggestions. Funding for this research was provided by the U.S. Department of Energy's (DOE) Atmospheric System Research (ASR) program and by the Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by DOE's Office of Biological and Environmental Research and located at PNNL. Pacific Northwest National Laboratory is operated for the U.S. Department of Energy by Battelle Memorial Institute under contract DE-AC06-76RLO1830. NR 75 TC 13 Z9 14 U1 1 U2 1 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD OCT 27 PY 2013 VL 118 IS 20 BP 11741 EP 11749 DI 10.1002/jgrd.50767 PG 9 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA V45WS UT WOS:000209847300020 ER PT J AU Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, C Rohringer, H Schofbeck, R Strauss, J Taurok, A Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, M Bansal, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Luyckx, S Mucibello, L Ochesanu, S Roland, B Rougny, R Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Kalogeropoulos, A Keaveney, J Maes, M Olbrechts, A Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Clerbaux, B De Lentdecker, G Favart, L Gay, APR Hreus, T Leonard, A Marage, PE Mohammadi, A Pernie, L Reis, T Seva, T Thomas, L Vander Velde, C Vanlaer, P Wang, J Adler, V Beernaert, K Benucci, L Cimmino, A Costantini, S Dildick, S Garcia, G Klein, B Lellouch, J Marinov, A Mccartin, J Rios, AAO Ryckbosch, D Sigamani, M Strobbe, N Thyssen, F Tytgat, M Walsh, S Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bruno, G Castello, R Caudron, A Ceard, L Delaere, C du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Lemaitre, V Liao, J Militaru, O Nuttens, C Pagano, D Pin, A Piotrzkowski, K Popov, A Selvaggi, M Garcia, JMV Beliy, N Caebergs, T Daubie, E Hammad, GH Alves, GA Martins, MC Martins, T Pol, ME Souza, MHG Alda, WL Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD De Souza, SF Malbouisson, H Malek, M Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santoro, A Jorge, LS Sznajder, A Manganote, EJT Pereira, AV Anjos, TS Bernardes, CA Dias, FA Tomei, TRFP Gregores, EM Lagana, C Marinho, F Mercadante, PG Novaes, SF Padula, SS Genchev, V Iaydjiev, P Piperov, S Rodozov, M Sultanov, G Vutova, M Dimitrov, A Hadjiiska, R Kozhuharov, V Litov, L Pavlov, B Petkov, P Bian, JG Chen, GM Chen, HS Jiang, CH Liang, D Liang, S Meng, X Tao, J Wang, J Wang, X Wang, Z Xiao, H Xu, M Asawatangtrakuldee, C Ban, Y Guo, Y Li, Q Li, W Liu, S Mao, Y Qian, S Wang, D Zhang, L Zou, W Avila, C Montoya, CAC Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Plestina, R Polic, D Puljak, I Antunovic, Z Kovac, M Brigljevic, V Duric, S Kadija, K Luetic, J Mekterovic, D Morovic, S Tikvica, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Finger, M Finger, M Assran, Y Kamel, AE Mahmoud, MA Mahrous, A Radi, A Kadastik, M Muntel, M Murumaa, M Raidal, M Rebane, L Tiko, A Eerola, P Fedi, G Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Kortelainen, MJ Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E Wendland, L Korpela, A Tuuva, T Besancon, M Choudhury, S Couderc, F Dejardin, M Denegri, D Fabbro, B Faure, JL Ferri, F Ganjour, S Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Malcles, J Millischer, L Nayak, A Rander, J Rosowsky, A Titov, M Baffioni, S Beaudette, F Benhabib, L Bianchini, L Bluj, M Busson, P Charlot, C Daci, N Dahms, T Dalchenko, M Dobrzynski, L Florent, A de Cassagnac, RG Haguenauer, M Mine, P Mironov, C Naranjo, I Nguyen, M Ochando, C Paganini, P Sabes, D Salerno, R Sirois, Y Veelken, C Zabi, A Agram, JL Andrea, J Bloch, D Bodin, D Brom, JM Chabert, EC Collard, C Conte, E Drouhin, F Fontaine, JC Gele, D Goerlach, U Goetzmann, C Juillot, P Le Bihan, AC Van Hove, P Gadrat, S Beauceron, S Beaupere, N Boudoul, G Brochet, S Chasserat, J Chierici, R Contardo, D Depasse, P El Mamouni, H Fay, J Gascon, S Gouzevitch, M Ille, B Kurca, T Lethuillier, M Mirabito, L Perries, S Sgandurra, L Sordini, V Tschudi, Y Vander Donckt, M Verdier, P Viret, S Tsamalaidze, Z Autermann, C Beranek, S 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Oberst, O Ott, J Quast, G Rabbertz, K Ratnikov, F Rocker, S Schilling, FP Schott, G Simonis, HJ Stober, FM Ulrich, R Wagner-Kuhr, J Wayand, S Weiler, T Zeise, M Anagnostou, G Daskalakis, G Geralis, T Kesisoglou, S Kyriakis, A Loukas, D Markou, A Markou, C Ntomari, E Gouskos, L Mertzimekis, TJ Panagiotou, A Saoulidou, N Stiliaris, E Aslanoglou, X Evangelou, I Flouris, G Foudas, C Kokkas, P Manthos, N Papadopoulos, I Paradas, E Bencze, G Hajdu, C Hidas, P Horvath, D Radics, B Sikler, F Veszpremi, V Vesztergombi, G Zsigmond, AJ Beni, N Czellar, S Molnar, J Palinkas, J Szillasi, Z Karancsi, J Raics, P Trocsanyi, ZL Ujvari, B Swain, SK Beri, SB Bhatnagar, V Dhingra, N Gupta, R Kaur, M Mehta, MZ Mittal, M Nishu, N Saini, LK Sharma, A Singh, JB Kumar, A Kumar, A Ahuja, S Bhardwaj, A Choudhary, BC Malhotra, S Naimuddin, M Ranjan, K Saxena, P Sharma, V Shivpuri, RK Banerjee, S Bhattacharya, S Chatterjee, K Dutta, S Gomber, B Jain, S Jain, S Khurana, R Modak, A Mukherjee, S Roy, D Sarkar, S 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CA CMS Collaboration TI Measurement of the W+W- cross section in pp collisions at and limits on anomalous WW gamma and WWZ couplings SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID GAUGE-BOSON COUPLINGS; PARTON DISTRIBUTIONS; ATLAS DETECTOR; ROOT-S=7 TEV; HIGGS-BOSON; LHC; SEARCH; LEP AB A measurement of W+W- production in pp collisions at is presented. The data were collected with the CMS detector at the LHC, and correspond to an integrated luminosity of 4.92 +/- 0.11 fb(-1). The W+W- candidates consist of two oppositely charged leptons, electrons or muons, accompanied by large missing transverse energy. The W+W- production cross section is measured to be 52.4 +/- 2.0 (stat.)+/- 4.5 (syst.)+/- 1.2 (lum.) pb. This measurement is consistent with the standard model prediction of 47.0 +/- 2.0 pb at next-to-leading order. Stringent limits on the WW gamma and WWZ anomalous triple gauge-boson couplings are set. C1 [Chatrchyan, S.; Khachatryan, V.; Sirunyan, A. 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[Albergo, S.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gallo, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Fabbri, F.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Fabbricatore, P.; Musenich, R.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Tosi, S.] Univ Genoa, Genoa, Italy. [Benaglia, A.; De Guio, F.; Di Matteo, L.; Fiorendi, S.; Gennai, S.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Massironi, A.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. 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T.; Montecassiano, F.; Passaseo, M.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Vanini, S.; Zotto, P.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Bellan, P.; Bisello, D.; Branca, A.; Carlin, R.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Vanini, S.; Zotto, P.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.; Lazzizzera, I.] Univ Trento Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Nappi, A.; Romeo, F.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Biasini, M.; Fano, L.; Lariccia, P.; Mantovani, G.; Nappi, A.; Romeo, F.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Boccali, T.; Broccolo, G.; Castaldi, R.; D'Agnolo, R. T.; Dell'Orso, R.; Fiori, F.; Foa, L.; Giassi, A.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; D'Agnolo, R. T.; Fiori, F.; Foa, L.; Ligabue, F.; Vernieri, C.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Diemoz, M.; Fanelli, C.; Grassi, M.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Soffi, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; Del Re, D.; Fanelli, C.; Grassi, M.; Longo, E.; Margaroli, F.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Soffi, L.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Dellacasa, G.; Demaria, N.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Pastrone, N.; Pelliccioni, M.; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Casasso, S.; Costa, M.; Migliore, E.; Monaco, V.; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Montanino, D.; Penzo, A.; Schizzi, A.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Kim, T. Y.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Chang, S.; Kim, D. H.; Kim, G. N.; Kim, J. E.; Kong, D. J.; Oh, Y. D.; Park, H.; Son, D. C.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, J. Y.; Kim, Z. J.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, T. J.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. S.; Kwon, E.; Lee, B.; Lee, J.; Lee, S.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Grigelionis, I.; Juodagalvis, A.] Vilnius Univ, Vilnius, Lithuania. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Lopez-Fernandez, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.; Reyes-Santos, M. A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Bell, A. J.; Butler, P. H.; Doesburg, R.; Reucroft, S.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Asghar, M. I.; Butt, J.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Wolszczak, W.] Univ Warsaw, Fac Phys, Inst Expt Phys, Warsaw, Poland. [Almeida, N.; Bargassa, P.; David, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Rodrigues Antunes, J.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Evstyukhin, S.; Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Erofeeva, M.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Markina, A.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia. [Adzic, P.; Ekmedzic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Aguilar-Benitez, M.; Alcaraz Maestre, J.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Navarro De Martino, E.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.; Willmott, C.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain. [Albajar, C.; de Trocniz, J. F.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.; Piedra Gomez, J.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Chuang, S. H.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Graziano, A.; Jorda, C.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Bendavid, J.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Perez, J. A. Coarasa; Colafranceschi, S.; d'Enterria, D.; Dabrowski, A.; De Roeck, A.; De Visscher, S.; Di Guida, S.; Dobson, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Funk, W.; Georgiou, G.; Giffels, M.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Giunta, M.; Glege, F.; Garrido, R. Gomez-Reino; Gowdy, S.; Guida, R.; Hammer, J.; Hansen, M.; Harris, P.; Hartl, C.; Hegner, B.; Hinzmann, A.; Innocente, V.; Janot, P.; Karavakis, E.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lee, Y. -J.; Magini, N.; Malberti, M.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moser, R.; Mulders, M.; Musella, P.; Nesvold, E.; Orsini, L.; Cortezon, E. Palencia; Perez, E.; Perrozzi, L.; Petrilli, A.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Piparo, D.; Polese, G.; Quertenmont, L.; Racz, A.; Reece, W.; Rolandi, G.; Rovelli, C.; Rovere, M.; Sakulin, H.; Santanastasio, F.; Schaefer, C.; Schwick, C.; Segoni, I.; Sekmen, S.; Sharma, A.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Stoye, M.; Tsirou, A.; Veres, G. I.; Vlimant, J. R.; Woehri, H. K.; Worm, S. D.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Gabathuler, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bortignon, P.; Buchmann, M. A.; Casal, B.; Chanon, N.; Deisher, A.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eller, P.; Grab, C.; Hits, D.; Lecomte, P.; Lustermann, W.; Marini, A. C.; del Arbol, P. Martinez Ruiz; Mohr, N.; Moortgat, F.; Naegeli, C.; Nef, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pape, L.; Pauss, F.; Peruzzi, M.; Ronga, F. J.; Rossini, M.; Sala, L.; Sanchez, A. K.; Starodumov, A.; Stieger, B.; Takahashi, M.; Tauscher, L.; Thea, A.; Theofilatos, K.; Treille, D.; Urscheler, C.; Wallny, R.; Weber, H. A.] ETH, Inst Particle Phys, Zurich, Switzerland. [Amsler, C.; Chiochia, V.; Favaro, C.; Rikova, M. Ivova; Kilminster, B.; Mejias, B. Millan; Otiougova, P.; Robmann, P.; Snoek, H.; Taroni, S.; Tupputi, S.; Verzetti, M.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Li, S. W.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Dietz, C.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Suwonjandee, N.] Chulalongkorn Univ, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Karapinar, G.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey. [Bahtiyar, H.; Barlas, E.; Cankocak, K.; Gunaydin, Y. O.; Vardarli, F. I.; Yucel, M.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Kreczko, L.; Metson, S.; Newbold, D. M.; Nirunpong, K.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Basso, L.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Jackson, J.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Womersley, W. J.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.; Whyntie, T.] Univ London Imperial Coll Sci Technol & Med, London, England. [Chadwick, M.; Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; St John, J.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Bhattacharya, S.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Houtz, R.; Ko, W.; Kopecky, A.; Lander, R.; Mall, O.; Miceli, T.; Nelson, R.; Pellett, D.; Ricci-Tam, F.; Rutherford, B.; Searle, M.; Smith, J.; Squires, M.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Andreev, V.; Cline, D.; Cousins, R.; Erhan, S.; Everaerts, P.; Farrell, C.; Felcini, M.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Rakness, G.; Schlein, P.; Takasugi, E.; Traczyk, P.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Babb, J.; Clare, R.; Dinardo, M. E.; Ellison, J.; Gary, J. W.; Hanson, G.; Liu, H.; Long, O. R.; Luthra, A.; Nguyen, H.; Paramesvaran, S.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; Evans, D.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Macneill, I.; Mangano, B.; Padhi, S.; Palmer, C.; Petrucciani, G.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, San Diego, CA 92103 USA. [Barge, D.; Bellan, R.; Campagnari, C.; D'Alfonso, M.; Danielson, T.; Flowers, K.; Geffert, P.; George, C.; Golf, F.; Incandela, J.; Justus, C.; Kalavase, P.; Kovalskyi, D.; Krutelyov, V.; Lowette, S.; Villalba, R. Magana; Mccoll, N.; Pavlunin, V.; Ribnik, J.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Di Marco, E.; Duarte, J.; Kcira, D.; Ma, Y.; Mott, A.; Newman, H. B.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Veverka, J.; Wilkinson, R.; Xie, S.; Yang, Y.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Liu, Y. F.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Eggert, N.; Gibbons, L. K.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Gutsche, O.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Klima, B.; Kunori, S.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Ratnikova, N.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Wu, W.; Yang, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Chen, M.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Drozdetskiy, A.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Remington, R.; Rinkevicius, A.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Hewamanage, S.; Lebolo, L. M.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Gleyzer, S. V.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Callner, J.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Lacroix, F.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Strom, D.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Griffiths, S.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Newsom, C. R.; Ogul, H.; Onel, Y.; Ozok, F.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Giurgiu, G.; Gritsan, A. V.; Hu, G.; Maksimovic, P.; Swartz, M.; Whitbeck, A.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Kenny, R. P., III; Murray, M.; Noonan, D.; Sanders, S.; Stringer, R.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Peterman, A.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Bauer, G.; Busza, W.; Butz, E.; Cali, I. A.; Chan, M.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Kim, Y.; Klute, M.; Lai, Y. S.; Levin, A.; Luckey, P. D.; Ma, T.; Nahn, S.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Sung, K.; Velicanu, D.; Wolf, R.; Wyslouch, B.; Yang, M.; Yilmaz, Y.; Yoon, A. S.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; De Benedetti, A.; Franzoni, G.; Gude, A.; Haupt, J.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Sasseville, M.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Cremaldi, L. M.; Kroeger, R.; Perera, L.; Rahmat, R.; Sanders, D. A.; Summers, D.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Eads, M.; Suarez, R. Gonzalez; Keller, J.; Kravchenko, I.; Lazo-Flores, J.; Malik, S.; Meier, F.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Dolen, J.; Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Kumar, A.; Rappoccio, S.; Wan, Z.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Nash, D.; Orimoto, T.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Anastassov, A.; Hahn, K. A.; Kubik, A.; Lusito, L.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Berry, D.; Brinkerhoff, A.; Chan, K. M.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kolb, J.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Morse, D. M.; Pearson, T.; Planer, M.; Ruchti, R.; Slaunwhite, J.; Valls, N.; Wayne, M.; Wolf, M.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Bylsma, B.; Durkin, L. S.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Puigh, D.; Rodenburg, M.; Smith, G.; Vuosalo, C.; Williams, G.; Winer, B. L.; Wolfe, H.] Ohio State Univ, Columbus, OH 43210 USA. [Berry, E.; Elmer, P.; Halyo, V.; Hebda, P.; Hegeman, J.; Hunt, A.; Jindal, P.; Koay, S. A.; Pegna, D. Lopes; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Raval, A.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zenz, S. C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Brownson, E.; Lopez, A.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA. [Alagoz, E.; Benedetti, D.; Bolla, G.; Bortoletto, D.; De Mattia, M.; Everett, A.; Hu, Z.; Jones, M.; Jung, K.; Koybasi, O.; Kress, M.; Leonardo, N.; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Marono, M. Vidal; Wang, F.; Xu, L.; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Guragain, S.; Parashar, N.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Ecklund, K. M.; Geurts, F. J. M.; Li, W.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; Covarelli, R.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Miner, D. C.; Petrillo, G.; Vishnevskiy, D.; Zielinski, M.] Univ Rochester, Rochester, NY 14627 USA. [Bhatti, A.; Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Malik, S.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Lath, A.; Panwalkar, S.; Park, M.; Patel, R.; Rekovic, V.; Robles, J.; Rose, K.; Salur, S.; Schnetzer, S.; Seitz, C.; Somalwar, S.; Stone, R.; Thomas, S.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Cerizza, G.; Hollingsworth, M.; Spanier, S.; Yang, Z. C.; York, A.] Univ Tennessee, Knoxville, TN USA. [Bouhali, O.; Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Khotilovich, V.; Montalvo, R.; Osipenkov, I.; Pakhotin, Y.; Perloff, A.; Roe, J.; Safonov, A.; Sakuma, T.; Suarez, I.; Tatarinov, A.; Toback, D.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Jeong, C.; Kovitanggoon, K.; Lee, S. W.; Libeiro, T.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Johns, W.; Maguire, C.; Mao, Y.; Melo, A.; Sharma, M.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN 37235 USA. [Arenton, M. W.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Lin, C.; Neu, C.; Wood, J.] Univ Virginia, Charlottesville, VA USA. [Gollapinni, S.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sakharov, A.] Wayne State Univ, Detroit, MI USA. [Anderson, M.; Belknap, D. A.; Borrello, L.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Friis, E.; Grogg, K. S.; Grothe, M.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Kaadze, K.; Klabbers, P.; Klukas, J.; Lanaro, A.; Lazaridis, C.; Loveless, R.; Mohapatra, A.; Mozer, M. U.; Ojalvo, I.; Pierro, G. A.; Ross, I.; Savin, A.; Smith, W. H.; Swanson, J.] Univ Wisconsin, Madison, WI 53706 USA. [Fabjan, C.; Fruehwirth, R.; Jeitler, M.; Krammer, M.; Wulz, C. -E.] Vienna Univ Technol, A-1040 Vienna, Austria. [Chinellato, J.; Tonelli Manganote, E. J.] Univ Estadual Campinas, Campinas, Brazil. [Assran, Y.] Suez Canal Univ, Suez, Egypt. [Kamel, A. Ellithi] Cairo Univ, Cairo, Egypt. [Mahmoud, M. A.] Fayoum Univ, Al Fayyum, Egypt. [Mahrous, A.] Helwan Univ, Cairo, Egypt. [Radi, A.] British Univ Egypt, Cairo, Egypt. [Radi, A.] Ain Shams Univ, Cairo, Egypt. [Agram, J. -L.; Conte, E.; Drouhin, F.; Fontaine, J. -C.] Univ Haute Alsace, Mulhouse, France. [Bergholz, M.; Lohmann, W.; Schmidt, R.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Vesztergombi, G.; Veres, G. I.] Eotvos Lorand Univ, Budapest, Hungary. [Gurtu, A.] King Abdulaziz Univ, Jeddah 21413, Saudi Arabia. [Maity, M.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka. [Arfaei, H.; Fahim, A.] Sharif Univ Technol, Tehran, Iran. [Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Safarzadeh, B.] Islamic Azad Univ, Sci & Res Branch, Plasma Phys Res Ctr, Tehran, Iran. [Androsov, K.; Martini, L.] Univ Siena, I-53100 Siena, Italy. [Heredia-de La Cruz, I.] Univ Michoacana, Morelia, Michoacan, Mexico. [Colafranceschi, S.] Univ Rome, Fac Ingn, Rome, Italy. [Rolandi, G.] Scuola Normale Super Pisa, Ist Nazl Fis Nucl, Pisa, Italy. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Bakirci, M. N.; Ozturk, S.; Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey. [Cerci, S.; Cerci, D. Sunar; Tali, B.] Adiyaman Univ, Adiyaman, Turkey. [Onengut, G.] Cag Univ, Mersin, Turkey. [Sogut, K.] Mersin Univ, Mersin, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Kaya, M.; Kaya, O.] Kafkas Univ, Kars, Turkey. [Ozkorucuklu, S.] Suleyman Demirel Univ, TR-32200 Isparta, Turkey. [Sonmez, N.] Ege Univ, Izmir, Turkey. [Bahtiyar, H.; Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Gunaydin, Y. O.] Kahramanmaras Sutcu Imam Univ, TR-46050 Kahramanmaras, Turkey. [Belyaev, A.; Basso, L.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Wasserbaech, S.] Utah Valley Univ, Orem, UT USA. [Bilki, B.] Argonne Natl Lab, Argonne, IL 60439 USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Yetkin, T.] Yildiz Tech Univ, Istanbul, Turkey. [Bouhali, O.] Texas A&M Univ Qatar, Doha, Qatar. [Kamon, T.] Kyungpook Natl Univ, Taegu, South Korea. [Adzic, P.; Ekmedzic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. RP Chatrchyan, S (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Mundim, Luiz/A-1291-2012; Haj Ahmad, Wael/E-6738-2016; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Ruiz, Alberto/E-4473-2011; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Andreev, Vladimir/M-8665-2015; TUVE', Cristina/P-3933-2015; KIM, Tae Jeong/P-7848-2015; Azarkin, Maxim/N-2578-2015; Flix, Josep/G-5414-2012; Della Ricca, Giuseppe/B-6826-2013; Tomei, Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Paganoni, Marco/A-4235-2016; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Tinoco Mendes, Andre David/D-4314-2011; Stahl, Achim/E-8846-2011; Trocsanyi, Zoltan/A-5598-2009; Konecki, Marcin/G-4164-2015; Hernandez Calama, Jose Maria/H-9127-2015; Bedoya, Cristina/K-8066-2014; My, Salvatore/I-5160-2015; Matorras, Francisco/I-4983-2015; Ragazzi, Stefano/D-2463-2009; Rovelli, Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Leonidov, Andrey/M-4440-2013; Benussi, Luigi/O-9684-2014; Russ, James/P-3092-2014; Leonidov, Andrey/P-3197-2014; vilar, rocio/P-8480-2014; da Cruz e Silva, Cristovao/K-7229-2013; Grandi, Claudio/B-5654-2015; Chinellato, Jose Augusto/I-7972-2012; Bernardes, Cesar Augusto/D-2408-2015; Raidal, Martti/F-4436-2012; Lazzizzera, Ignazio/E-9678-2015; Sen, Sercan/C-6473-2014; D'Alessandro, Raffaello/F-5897-2015; Belyaev, Alexander/F-6637-2015; Cerrada, Marcos/J-6934-2014; Venturi, Andrea/J-1877-2012; Calderon, Alicia/K-3658-2014; de la Cruz, Begona/K-7552-2014; Scodellaro, Luca/K-9091-2014; Josa, Isabel/K-5184-2014; Calvo Alamillo, Enrique/L-1203-2014; VARDARLI, Fuat Ilkehan/B-6360-2013; Manganote, Edmilson/K-8251-2013; Paulini, Manfred/N-7794-2014; Vogel, Helmut/N-8882-2014; Ferguson, Thomas/O-3444-2014; Wolszczak, Weronika/N-3113-2013; Montanari, Alessandro/J-2420-2012; Gribushin, Andrei/J-4225-2012; Petrushanko, Sergey/D-6880-2012; Marlow, Daniel/C-9132-2014; de Jesus Damiao, Dilson/G-6218-2012; Janssen, Xavier/E-1915-2013; Novaes, Sergio/D-3532-2012; Bartalini, Paolo/E-2512-2014; Ligabue, Franco/F-3432-2014; Wulz, Claudia-Elisabeth/H-5657-2011; Dudko, Lev/D-7127-2012; Lokhtin, Igor/D-7004-2012 OI Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Mundim, Luiz/0000-0001-9964-7805; Haj Ahmad, Wael/0000-0003-1491-0446; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; Flix, Josep/0000-0003-2688-8047; Della Ricca, Giuseppe/0000-0003-2831-6982; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Paganoni, Marco/0000-0003-2461-275X; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Stahl, Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279; Konecki, Marcin/0000-0001-9482-4841; Hernandez Calama, Jose Maria/0000-0001-6436-7547; Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680; Matorras, Francisco/0000-0003-4295-5668; Ragazzi, Stefano/0000-0001-8219-2074; Rovelli, Tiziano/0000-0002-9746-4842; Benussi, Luigi/0000-0002-2363-8889; Russ, James/0000-0001-9856-9155; Grandi, Claudio/0000-0001-5998-3070; Chinellato, Jose Augusto/0000-0002-3240-6270; Lazzizzera, Ignazio/0000-0001-5092-7531; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Belyaev, Alexander/0000-0002-1733-4408; Cerrada, Marcos/0000-0003-0112-1691; Scodellaro, Luca/0000-0002-4974-8330; Calvo Alamillo, Enrique/0000-0002-1100-2963; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Ferguson, Thomas/0000-0001-5822-3731; Montanari, Alessandro/0000-0003-2748-6373; de Jesus Damiao, Dilson/0000-0002-3769-1680; Novaes, Sergio/0000-0003-0471-8549; Ligabue, Franco/0000-0002-1549-7107; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Dudko, Lev/0000-0002-4462-3192; FU BMWF (Austria); FWF (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MEYS (Bulgaria); CERN; CAS (China); MoST (China); NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); MoER [SF0690030s09]; ERDF (Estonia); Academy of Finland (Finland); MEC (Finland); HIP (Finland); CEA (France); CNRS/IN2P3 (France); BMBF (Germany); DFG (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NKTH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF (Republic of Korea); WCU (Republic of Korea); LAS (Lithuania); CINVESTAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); MSI (New Zealand); PAEC (Pakistan); MSHE (Poland); NSC (Poland); FCT (Portugal); JINR (Armenia); JINR (Belarus); JINR (Georgia); JINR (Ukraine); JINR (Uzbekistan); MON (Russia); RosAtom (Russia); RAS (Russia); RFBR (Russia); MSTD (Serbia); SEIDI (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); ThEPCenter (Thailand); IPST (Thailand); NSTDA (Thailand); TUBITAK (Turkey); TAEK (Turkey); NASU (Ukraine); STFC (United Kingdom); DOE (USA); NSF (USA); Marie-Curie programme; European Research Council; EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of Czech Republic; Council of Science and Industrial Research, India; Compagnia di San Paolo (Torino); HOMING PLUS programme of Foundation for Polish Science; EU, Regional Development Fund; Thalis programme; Aristeia programme; EU-ESF; Greek NSRF FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centres and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWF and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MEYS (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); MoER, SF0690030s09 and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NKTH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF and WCU (Republic of Korea); LAS (Lithuania); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MSI (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Armenia, Belarus, Georgia, Ukraine, Uzbekistan); MON, RosAtom, RAS and RFBR (Russia); MSTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); ThEPCenter, IPST and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU (Ukraine); STFC (United Kingdom); DOE and NSF (USA).; Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of Czech Republic; the Council of Science and Industrial Research, India; the Compagnia di San Paolo (Torino); the HOMING PLUS programme of Foundation for Polish Science, cofinanced by EU, Regional Development Fund; and the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF. NR 48 TC 22 Z9 22 U1 4 U2 107 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD OCT 26 PY 2013 VL 73 IS 10 AR 2610 DI 10.1140/epjc/s10052-013-2610-8 PG 22 WC Physics, Particles & Fields SC Physics GA 244KE UT WOS:000326386200001 ER PT J AU Kilgore, WB AF Kilgore, William B. TI The two-loop infrared structure of amplitudes with mixed gauge groups SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID JET CROSS-SECTIONS; QCD CORRECTIONS; GLUON SCATTERING; ORDER; QUARK; ALGORITHM AB The infrared structure of (multi-loop) scattering amplitudes is determined entirely by the identities of the external particles participating in the scattering. The two-loop infrared structure of pure QCD amplitudes has been known for some time. By computing the two-loop amplitudes for (f) over barf -> X and (f) over barf -> V1V2 scattering in an SU(N) x SU(M) x U(1) gauge theory, I determine the anomalous dimensions which govern the infrared structure for any massless two-loop amplitude. C1 Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. RP Kilgore, WB (reprint author), Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. EM kilgore@bnl.gov FU U.S. Department of Energy [DE-AC02-98CH10886] FX This research was supported by the U.S. Department of Energy under Contract No. DE-AC02-98CH10886. NR 39 TC 0 Z9 0 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD OCT 25 PY 2013 VL 73 IS 10 AR 2603 DI 10.1140/epjc/s10052-013-2603-7 PG 8 WC Physics, Particles & Fields SC Physics GA AC0JC UT WOS:000332179600001 ER PT J AU Li, CL Tanjore, D He, W Wong, J Gardner, JL Sale, KL Simmons, BA Singh, S AF Li, Chenlin Tanjore, Deepti He, Wei Wong, Jessica Gardner, James L. Sale, Kenneth L. Simmons, Blake A. Singh, Seema TI Scale-up and evaluation of high solid ionic liquid pretreatment and enzymatic hydrolysis of switchgrass SO BIOTECHNOLOGY FOR BIOFUELS LA English DT Article DE Scale-up; Pretreatment; Saccharification; Ionic liquid; High solid loading; Viscosity; Inhibition ID WHEAT-STRAW; DILUTE-ACID; CORN STOVER; LIGNOCELLULOSIC BIOMASS; SACCHARIFICATION; EXTRACTION; LIGNIN; SUGARS; RECALCITRANCE; FERMENTATION AB Background: Ionic liquid (IL) pretreatment is receiving significant attention as a potential process that enables fractionation of lignocellulosic biomass and produces high yields of fermentable sugars suitable for the production of renewable fuels. However, successful optimization and scale up of IL pretreatment involves challenges, such as high solids loading, biomass handling and transfer, washing of pretreated solids and formation of inhibitors, which are not addressed during the development stages at the small scale in a laboratory environment. As a first in the research community, the Joint BioEnergy Institute, in collaboration with the Advanced Biofuels Process Demonstration Unit, a Department of Energy funded facility that supports academic and industrial entities in scaling their novel biofuels enabling technologies, have performed benchmark studies to identify key challenges associated with IL pretreatment using 1-ethyl-3-methylimidazolium acetate and subsequent enzymatic saccharification beyond bench scale. Results: Using switchgrass as the model feedstock, we have successfully executed 600-fold, relative to the bench scale (6 L vs 0.01 L), scale-up of IL pretreatment at 15% (w/w) biomass loading. Results show that IL pretreatment at 15% biomass generates a product containing 87.5% of glucan, 42.6% of xylan and only 22.8% of lignin relative to the starting material. The pretreated biomass is efficiently converted into monosaccharides during subsequent enzymatic hydrolysis at 10% loading over a 150-fold scale of operations (1.5 L vs 0.01 L) with 99.8% fermentable sugar conversion. The yield of glucose and xylose in the liquid streams were 94.8% and 62.2%, respectively, and the hydrolysate generated contains high titers of fermentable sugars (62.1 g/L of glucose and 5.4 g/L cellobiose). The overall glucan and xylan balance from pretreatment and saccharification were 95.0% and 77.1%, respectively. Enzymatic inhibition by [C(2)mim][OAc] at high solids loadings requires further process optimization to obtain higher yields of fermentable sugars. Conclusion: Results from this initial scale up evaluation indicate that the IL-based conversion technology can be effectively scaled to larger operations and the current study establishes the first scaling parameters for this conversion pathway but several issues must be addressed before a commercially viable technology can be realized, most notably reduction in water consumption and efficient IL recycle. C1 [Li, Chenlin; Tanjore, Deepti; He, Wei; Wong, Jessica; Gardner, James L.] Lawrence Berkeley Natl Lab, Adv Biofuels Proc Demonstrat Unit, Emeryville, CA USA. [Sale, Kenneth L.; Simmons, Blake A.; Singh, Seema] Joint BioEnergy Inst, Deconstruct Div, Emeryville, CA USA. [Sale, Kenneth L.; Simmons, Blake A.; Singh, Seema] Sandia Natl Labs, Biol & Mat Sci Ctr, Livermore, CA USA. RP Singh, S (reprint author), Joint BioEnergy Inst, Deconstruct Div, Emeryville, CA USA. EM seesing@sandia.gov OI Li, Chenlin/0000-0002-0793-0505 FU Office of Biomass Program within the US DOE's Office of Energy Efficiency and Renewable Energy; American Recovery and Reinvestment Act; US DOE's Office of Science, Office of Biological and Environmental Research [DE-AC02-05CH11231] FX ABPDU would like to acknowledge the funding support from Office of Biomass Program within the US DOE's Office of Energy Efficiency and Renewable Energy, and also the funding support from the American Recovery and Reinvestment Act. JBEI would like to acknowledge the funding support from US DOE's Office of Science, Office of Biological and Environmental Research, through contract DE-AC02-05CH11231 between Lawrence Berkeley National Laboratory and the US DOE. The authors would like to thank the Laboratory of Dr. Daniel Putnam from the University of California at Davis for providing the switchgrass, and Novozymes for the gift of the enzyme cocktails used in this work. NR 52 TC 21 Z9 21 U1 6 U2 73 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1754-6834 J9 BIOTECHNOL BIOFUELS JI Biotechnol. Biofuels PD OCT 25 PY 2013 VL 6 AR 154 DI 10.1186/1754-6834-6-154 PG 13 WC Biotechnology & Applied Microbiology; Energy & Fuels SC Biotechnology & Applied Microbiology; Energy & Fuels GA 247WH UT WOS:000326653100001 PM 24160440 ER PT J AU Rao, RR Roberts, SA Noble, DR Anderson, PD Hetu, JF AF Rao, Rekha R. Roberts, S. A. Noble, David R. Anderson, Patrick D. Hetu, Jean-Francois TI USNCCM-11: Computational fluid mechanics for free and moving boundary problems SO COMPUTERS & FLUIDS LA English DT Editorial Material C1 [Rao, Rekha R.; Roberts, S. A.; Noble, David R.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Anderson, Patrick D.] Eindhoven Univ Technol, NL-5600 MB Eindhoven, Netherlands. [Hetu, Jean-Francois] Natl Res Council Canada, Boucherville, PQ J4B 6Y4, Canada. RP Rao, RR (reprint author), Sandia Natl Labs, MS 0836, Albuquerque, NM 87185 USA. EM rrrao@sandia.gov RI Anderson, Patrick/E-6046-2011; OI Anderson, Patrick/0000-0001-9157-0858 NR 13 TC 0 Z9 0 U1 0 U2 7 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0045-7930 EI 1879-0747 J9 COMPUT FLUIDS JI Comput. Fluids PD OCT 25 PY 2013 VL 87 SI SI BP 1 EP 1 DI 10.1016/j.compfluid.2013.09.023 PG 1 WC Computer Science, Interdisciplinary Applications; Mechanics SC Computer Science; Mechanics GA 244AX UT WOS:000326360600001 ER PT J AU Roberts, SA Noble, DR Benner, EM Schunk, PR AF Roberts, Scott A. Noble, David R. Benner, Eric M. Schunk, P. Randall TI Multiphase hydrodynamic lubrication flow using a three-dimensional shell finite element model SO COMPUTERS & FLUIDS LA English DT Article DE Lubrication theory; Finite-element method; Shell elements; Level-set method; Multiphase flow ID THERMAL-ELASTOHYDRODYNAMIC LUBRICATION; FLASH IMPRINT LITHOGRAPHY; SLIDE-ROLL RATIOS; POWER-LAW FLUID; JOURNAL-BEARING; LEVEL SET; CONTACT SOLUTION; SURFACE-TENSION; 2-PHASE FLOWS; LINE CONTACT AB Reynolds' lubrication theory has been widely used to study thin-region fluid flows for a variety of scientific and manufacturing applications. In this work, we set forth an extension of this theory to model the effect of free fluid interfaces and fluid-structural interactions in lubrication films. This model is implemented using curvilinear shell elements in a general three-dimensional finite element code, allowing the study of lubrication flows in arbitrarily complex geometries. This implementation also allows coupling with continuum mechanics, such as solid body deformation, through lubrication-based and fluid-structural interactions. Simulations using this model are compared to analytical solutions and experimental results for a number of model problems. (C) 2012 Elsevier Ltd. All rights reserved. C1 [Roberts, Scott A.; Noble, David R.] Sandia Natl Labs, Thermal & Fluid Proc Dept, Albuquerque, NM 87185 USA. [Benner, Eric M.; Schunk, P. Randall] Sandia Natl Labs, Nanoscale & React Proc Dept, Albuquerque, NM 87185 USA. RP Roberts, SA (reprint author), Sandia Natl Labs, Thermal & Fluid Proc Dept, POB 5800,MS-0836, Albuquerque, NM 87185 USA. EM sarober@sandia.gov RI Roberts, Scott/C-1158-2009 OI Roberts, Scott/0000-0002-4196-6771 FU US Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors acknowledge Sandia National Laboratories' Laboratory Directed Research and Development program. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the US Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 76 TC 3 Z9 3 U1 1 U2 26 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0045-7930 EI 1879-0747 J9 COMPUT FLUIDS JI Comput. Fluids PD OCT 25 PY 2013 VL 87 SI SI BP 12 EP 25 DI 10.1016/j.compfluid.2012.08.009 PG 14 WC Computer Science, Interdisciplinary Applications; Mechanics SC Computer Science; Mechanics GA 244AX UT WOS:000326360600003 ER PT J AU Kapahi, A Sambasivan, S Udaykumar, HS AF Kapahi, A. Sambasivan, S. Udaykumar, H. S. TI Simulation of collapse and fragmentation phenomena in a sharp interface Eulerian setting SO COMPUTERS & FLUIDS LA English DT Article DE Eulerian; Sharp interface method; Level set method; Ghost Fluid Method (GFM); Void collapse; Fragmentation Least squares method ID GHOST FLUID METHOD; VOID COLLAPSE; MULTIMATERIAL FLOWS; ENERGETIC MATERIAL; LEVEL SET; PART 1; IMPACT; EXPLOSIVES; PENETRATION; SCHEMES AB Sharp interface Eulerian methods are used to develop a technique for handling high speed material dynamics leading to collapse and fragmentation. Two problems are of primary interest, viz, void collapse in energetic materials and fragmentation of solids under impact; in the first case the sharp interface reconnects to itself, while in the second the sharp interface is torn apart. The challenge is to simulate using a sharp interface Eulerian approach through these topological changes and to apply boundary conditions on the immersed interfaces. Level set interface representations are combined with a modified Ghost Fluid Method to solve sharp interface dynamics in the presence of elasto-plastically deforming solid materials. A unified method of populating ghost field is developed using an adaptive least squares approach and demonstrated to be robust for severe interface deformations, including changes in topology. A parallel algorithm is used to enable solutions of large scale problems. The embedded material interfaces undergoing severe deformation while moving at a very high speed are handled efficiently and accurately in a multi-processor setting. Validation exercises, examples and benchmark calculations are presented to demonstrate the accuracy of the approach. (C) 2012 Elsevier Ltd. All rights reserved. C1 [Kapahi, A.; Udaykumar, H. S.] Univ Iowa, Dept Mech & Ind Engn, Iowa City, IA 52242 USA. [Sambasivan, S.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Udaykumar, HS (reprint author), Univ Iowa, Dept Mech & Ind Engn, 3131 Seamans Ctr, Iowa City, IA 52242 USA. EM hs-kumar@uiowa.edu FU AFOSR; AFRL-RWPC (Computational Mechanics Branch, Eglin AFB) FX This work was performed under grants from the AFOSR Computational Mathematics program (Program Manager: Dr. Fariba Fahroo) and from the AFRL-RWPC (Computational Mechanics Branch, Eglin AFB, Program Manager: Dr. Michael E. Nixon). NR 48 TC 1 Z9 1 U1 1 U2 10 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0045-7930 EI 1879-0747 J9 COMPUT FLUIDS JI Comput. Fluids PD OCT 25 PY 2013 VL 87 SI SI BP 26 EP 40 DI 10.1016/j.compfluid.2012.09.007 PG 15 WC Computer Science, Interdisciplinary Applications; Mechanics SC Computer Science; Mechanics GA 244AX UT WOS:000326360600004 ER PT J AU Clausen, JR AF Clausen, Jonathan R. TI Using the suspension balance model in a finite-element flow solver SO COMPUTERS & FLUIDS LA English DT Article DE Suspensions; Suspension balance; Multiphase flow ID STOKESIAN DYNAMICS SIMULATION; COMPUTATIONAL FLUID-DYNAMICS; SHEAR-INDUCED MIGRATION; PRESSURE-DRIVEN FLOW; CONCENTRATED SUSPENSIONS; PARTICLE MIGRATION; NORMAL STRESSES; RIGID SPHERES; NONCOLLOIDAL SUSPENSIONS; COLLOIDAL SUSPENSIONS AB A suspension balance model (SBM) is implemented to describe the shear-driven migration of particles in noncolloidal suspensions in the context of a finite element (FE) solver. Before developing the FE methodology, the SBM is analyzed in the context of a rigorous two-phase averaging procedure, in which the traditional SBM model can be thought of as an approximate closure relationship for the rigorous two-phase equations. It is shown that the standard SBM equations are inconsistent, which is demonstrated analytically for the case of Couette flow. A FE model is developed using a corrected set of SBM equations, and the numerical techniques needed to handle the anisotropic Q-tensor and FE stabilization are detailed. The resultant FE-SBM method is tested using a Couette geometry and compared with existing models and experiments. A high level of sensitivity of the particle migration to the chosen viscosity model is noted, as well as the influence of excess diffusion caused by the FE stabilization procedure. The FE-SBM method is also used in conjunction with an arbitrary Lagrangian-Eulerian formulation to simulate the deflection of the free surface in a Couette cell. Secondary flows are observed in the free-surface simulation results, and the underlying mechanisms driving these secondary flows are explored. (C) 2013 Elsevier Ltd. All rights reserved. C1 Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Clausen, JR (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM jclause@sandia.gov FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 60 TC 2 Z9 2 U1 4 U2 9 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0045-7930 EI 1879-0747 J9 COMPUT FLUIDS JI Comput. Fluids PD OCT 25 PY 2013 VL 87 SI SI BP 67 EP 78 DI 10.1016/j.compfluid.2012.12.004 PG 12 WC Computer Science, Interdisciplinary Applications; Mechanics SC Computer Science; Mechanics GA 244AX UT WOS:000326360600008 ER PT J AU Francois, MM Carlson, NN AF Francois, Marianne M. Carlson, Neil N. TI The global embedded interface formulation for interfacial mass transfer within a volume tracking framework SO COMPUTERS & FLUIDS LA English DT Article DE Volume tracking; Mass transfer; Interfacial flow; Droplet dynamics ID NUMERICAL-SIMULATION; SURFACE-TENSION; FLOW; BUBBLES AB Interfacial flow with mass transfer is particularly challenging to compute because the position of the interface between the fluids and the interface physics needs to be predicted as part of the solution of the flow equations. In addition, the discontinuity in fluid density, viscosity and species concentration at the interface present additional numerical challenges. In this work, we extend our balanced-force volume-tracking algorithm for modeling interfacial flow with surface tension force [10] to include mass transfer. We propose a global embedded interface formulation to model the interfacial conditions of the species concentration at an interface in thermodynamic equilibrium. To verify our formulation, we perform simulations of a pure diffusion problem with species concentration discontinuity at the interface. Then we present two and three-dimensional simulations of droplets rising by buoyancy with mass transfer. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Francois, Marianne M.; Carlson, Neil N.] Los Alamos Natl Lab, Computat Phys & Methods Grp CCS 2, Los Alamos, NM 87545 USA. RP Francois, MM (reprint author), Los Alamos Natl Lab, Computat Phys & Methods Grp CCS 2, POB 1663, Los Alamos, NM 87545 USA. EM mmfran@lanl.gov OI Francois, Marianne/0000-0003-3062-6234 FU National Nuclear Security Administration of the US Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396]; Nuclear Energy Office of the Department of Energy FX This work was performed under the auspices of the National Nuclear Security Administration of the US Department of Energy at Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396. This work is supported by the Nuclear Energy Office of the Department of Energy. The authors thank Boonthanome Nouanesengsy and John Patchett of the paraview team for their help with post-processing the data for the nine droplets test cases and Matthew Wagner, summer student in CCS-2 for his help with the simulations presented in Section 5.1. NR 25 TC 2 Z9 2 U1 0 U2 5 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0045-7930 EI 1879-0747 J9 COMPUT FLUIDS JI Comput. Fluids PD OCT 25 PY 2013 VL 87 SI SI BP 102 EP 114 DI 10.1016/j.compfluid.2013.02.016 PG 13 WC Computer Science, Interdisciplinary Applications; Mechanics SC Computer Science; Mechanics GA 244AX UT WOS:000326360600011 ER PT J AU Li, G Zhang, Q Rhodes, D Zeng, B Goswami, P Baumbach, RE Tobash, PH Ronning, F Thompson, JD Bauer, ED Balicas, L AF Li, G. Zhang, Q. Rhodes, D. Zeng, B. Goswami, P. Baumbach, R. E. Tobash, P. H. Ronning, F. Thompson, J. D. Bauer, E. D. Balicas, L. TI Bulk evidence for a time-reversal symmetry broken superconducting state in URu2Si2 SO PHYSICAL REVIEW B LA English DT Article ID HIDDEN-ORDER; FIELD; EXCITATIONS; TRANSITION; LATTICE; WAVE AB URu2Si2 is claimed to be a chiral d-wave superconductor with a k(z) (k(x) +/- ik(y)) time-reversal symmetry broken orbital component for the Cooper pair wave function, which contains both nodal points and lines of nodes. To study the magnetic response of such an unconventional state through a bulk, thermodynamic probe, we measured the magnetic torque t in very high-quality, well-characterized URu2Si2 single crystals at high magnetic fields H and at very low temperatures T. The magnetization M(H) proportional to tau(H)/H of URu2Si2, in its superconducting state and for angles within 15. from the ab plane, reveals a change in its sign for H approaching H-c2: from a clear diamagnetic response dominated by the pinning of vortices to a state with a smaller but "paramagneticlike" hysteretic response which disappears at H-c2, thus implying that it is intrinsically related to the superconducting state. We argue that this anomalous, angular-dependent behavior is evidence for a time-reversal symmetry broken superconducting state in URu2Si2, although not necessarily for the k(z) (k(x) +/- ik(y)) state. C1 [Li, G.; Zhang, Q.; Rhodes, D.; Zeng, B.; Goswami, P.; Balicas, L.] Florida State Univ, Natl High Magnet Field Lab, Tallahassee, FL 32310 USA. [Baumbach, R. E.; Tobash, P. H.; Ronning, F.; Thompson, J. D.; Bauer, E. D.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Li, G (reprint author), Florida State Univ, Natl High Magnet Field Lab, Tallahassee, FL 32310 USA. EM balicas@magnet.fsu.edu RI Zeng, Bin/O-3370-2013; Rhodes, Daniel/H-3423-2013; Li, Gang/E-3033-2015; OI Zeng, Bin/0000-0002-0090-4371; Ronning, Filip/0000-0002-2679-7957; Bauer, Eric/0000-0003-0017-1937 FU NSF [NSF-DMR-0084173]; State of Florida; DOE-BES [DE-SC0002613]; US DOE, Office of Science FX We acknowledge discussions with N. Harrison. The NHMFL is supported by NSF through Grant No. NSF-DMR-0084173 and the State of Florida. L. B. is supported by DOE-BES through award DE-SC0002613. The work at the LANL is carried out under the auspices of the US DOE, Office of Science. NR 38 TC 13 Z9 13 U1 2 U2 20 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 25 PY 2013 VL 88 IS 13 AR 134517 DI 10.1103/PhysRevB.88.134517 PG 7 WC Physics, Condensed Matter SC Physics GA 240KK UT WOS:000326094500005 ER PT J AU Nisoli, C Abraham, D Lookman, T Saxena, A AF Nisoli, Cristiano Abraham, Douglas Lookman, Turab Saxena, Avadh TI Quasi-one-dimensional thermal breakage SO PHYSICAL REVIEW E LA English DT Article ID 2-DIMENSIONAL ISING-MODEL; SI(001) SURFACE; NANOWIRES; GROWTH; TRANSITION; MICROSCOPY; POLYMERS; DNA AB Breakage is generally understood in mechanical terms, yet nanostructures can rupture not only under external loads but also via thermal activation. Here we treat in a general framework the statistical mechanics of thermally induced breakage at the nanoscale for one-dimensional systems. We test it on a simple approximation and find that the probability of breakage controls distinct regimes, characterized by sharp crossovers and narrow peaks in the thermal fluctuations and specific heat. Our work provides predictions on clustering of new phases, of relevance in nanofabrication. C1 [Nisoli, Cristiano; Abraham, Douglas; Lookman, Turab; Saxena, Avadh] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Nisoli, Cristiano; Abraham, Douglas; Lookman, Turab; Saxena, Avadh] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. [Abraham, Douglas] Rudolf Peierls Ctr Theoret Phys, Oxford OX1 3NP, England. RP Nisoli, C (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. OI Nisoli, Cristiano/0000-0003-0053-1023 FU National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory [DEAC52-06NA25396] FX This work was carried out under the auspices of the National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory under Contract No. DEAC52-06NA25396. NR 34 TC 0 Z9 0 U1 0 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1539-3755 EI 1550-2376 J9 PHYS REV E JI Phys. Rev. E PD OCT 25 PY 2013 VL 88 IS 4 AR 042409 DI 10.1103/PhysRevE.88.042409 PG 7 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA 240SZ UT WOS:000326118600005 PM 24229191 ER PT J AU Brown, RS Deng, ZD Cook, KV Pflugrath, BD Li, XY Fu, T Martinez, JJ Li, HD Trumbo, BA Ahmann, ML Seaburg, AG AF Brown, Richard S. Deng, Z. Daniel Cook, Katrina V. Pflugrath, Brett D. Li, Xinya Fu, Tao Martinez, Jayson J. Li, Huidong Trumbo, Bradly A. Ahmann, Martin L. Seaburg, Adam G. TI A Field Evaluation of an External and Neutrally Buoyant Acoustic Transmitter for Juvenile Salmon: Implications for Estimating Hydroturbine Passage Survival SO PLOS ONE LA English DT Article ID HYDRO-TURBINE PASSAGE; CHINOOK SALMON; SWIMMING PERFORMANCE; SNAKE RIVER; COLUMBIA RIVER; TELEMETRY TRANSMITTERS; ATTACHED TRANSMITTERS; ANADROMOUS SALMONIDS; AVIAN PREDATION; SMALLMOUTH BASS AB Turbine-passed fish are exposed to rapid decreases in pressure which can cause barotrauma. The presence of an implanted telemetry tag increases the likelihood of injury or death from exposure to pressure changes, thus potentially biasing studies evaluating survival of turbine-passed fish. Therefore, a neutrally buoyant externally attached tag was developed to eliminate this bias in turbine passage studies. This new tag was designed not to add excess mass in water or take up space in the coelom, having an effective tag burden of zero with the goal of reducing pressure related biases to turbine survival studies. To determine if this new tag affects fish performance or susceptibility to predation, it was evaluated in the field relative to internally implanted acoustic transmitters (JSATS; Juvenile Salmon Acoustic Telemetry System) used widely for survival studies of juvenile salmonids. Survival and travel time through the study reach was compared between fish with either tag type in an area of high predation in the Snake and Columbia rivers, Washington. An additional group of fish affixed with neutrally-buoyant dummy external tags were implanted with passive integrated transponder (PIT) tags and recovered further downstream to assess external tag retention and injury. There were no significant differences in survival to the first detection site, 12 river kilometers (rkm) downstream of release. Travel times were also similar between groups. Conversely, externally-tagged fish had reduced survival (or elevated tag loss) to the second detection site, 65 rkm downstream. In addition, the retention study revealed that tag loss was first observed in fish recaptured approximately 9 days after release. Results suggest that this new tag may be viable for short term (< 8 days) single-dam turbine-passage studies and under these situations, may alleviate the turbine passage-related bias encountered when using internal tags, however further research is needed to confirm this. C1 [Brown, Richard S.; Cook, Katrina V.; Pflugrath, Brett D.] Pacific NW Natl Lab, Ecol Grp, Richland, WA 99352 USA. [Deng, Z. Daniel; Li, Xinya; Fu, Tao; Martinez, Jayson J.; Li, Huidong] Pacific NW Natl Lab, Hydrol Grp, Richland, WA 99352 USA. [Trumbo, Bradly A.; Ahmann, Martin L.] US Army, Corps Engineers, Walla Walla, WA USA. [Seaburg, Adam G.] Univ Washington, Sch Aquat & Fishery Sci, Seattle, WA 98195 USA. RP Brown, RS (reprint author), Pacific NW Natl Lab, Ecol Grp, Richland, WA 99352 USA. EM rich.brown@pnnl.gov RI Deng, Daniel/A-9536-2011 OI Deng, Daniel/0000-0002-8300-8766 FU U.S. Army corps of Engineers, Walla Walla district (Walla Walla Washington State) [W912EF-08-D-0004] FX This study was funded by the U.S. Army corps of Engineers, Walla Walla district (Walla Walla Washington State) under contract number W912EF-08-D-0004. Funders were involved in study design and preparation of the manuscript (authors BAT and MLA). NR 55 TC 3 Z9 3 U1 3 U2 25 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD OCT 25 PY 2013 VL 8 IS 10 AR e77744 DI 10.1371/journal.pone.0077744 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 241GW UT WOS:000326155400054 PM 24204947 ER PT J AU Reddy, AP Simmons, CW D'haeseleer, P Khudyakov, J Burd, H Hadi, M Simmons, BA Singer, SW Thelen, MP VanderGheynst, JS AF Reddy, Amitha P. Simmons, Christopher W. D'haeseleer, Patrik Khudyakov, Jane Burd, Helcio Hadi, Masood Simmons, Blake A. Singer, Steven W. Thelen, Michael P. VanderGheynst, Jean S. TI Discovery of Microorganisms and Enzymes Involved in High-Solids Decomposition of Rice Straw Using Metagenomic Analyses SO PLOS ONE LA English DT Article ID SP-NOV.; LIGNOCELLULOSIC BIOFUELS; KOREAN GINSENG; BINDING MODULE; GEN. NOV.; CELLULOSE; SOIL; COMMUNITY; RESOURCE; SYSTEM AB High-solids incubations were performed to enrich for microbial communities and enzymes that decompose rice straw under mesophilic (35 degrees C) and thermophilic (55 degrees C) conditions. Thermophilic enrichments yielded a community that was 7.5 times more metabolically active on rice straw than mesophilic enrichments. Extracted xylanase and endoglucanse activities were also 2.6 and 13.4 times greater, respectively, for thermophilic enrichments. Metagenome sequencing was performed on enriched communities to determine community composition and mine for genes encoding lignocellulolytic enzymes. Proteobacteria were found to dominate the mesophilic community while Actinobacteria were most abundant in the thermophilic community. Analysis of protein family representation in each metagenome indicated that cellobiohydrolases containing carbohydrate binding module 2 (CBM2) were significantly overrepresented in the thermophilic community. Micromonospora, a member of Actinobacteria, primarily housed these genes in the thermophilic community. In light of these findings, Micromonospora and other closely related Actinobacteria genera appear to be promising sources of thermophilic lignocellulolytic enzymes for rice straw deconstruction under high-solids conditions. Furthermore, these discoveries warrant future research to determine if exoglucanases with CBM2 represent thermostable enzymes tolerant to the process conditions expected to be encountered during industrial biofuel production. C1 [Reddy, Amitha P.; Simmons, Christopher W.; D'haeseleer, Patrik; Khudyakov, Jane; Burd, Helcio; Hadi, Masood; Simmons, Blake A.; Singer, Steven W.; Thelen, Michael P.; VanderGheynst, Jean S.] Joint BioEnergy Inst, Emeryville, CA USA. [Reddy, Amitha P.; Simmons, Christopher W.; VanderGheynst, Jean S.] Univ Calif Davis, Davis, CA 95616 USA. [Singer, Steven W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [D'haeseleer, Patrik; Khudyakov, Jane; Thelen, Michael P.] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA USA. [Hadi, Masood; Simmons, Blake A.] Sandia Natl Labs, Biol & Mat Sci Ctr, Livermore, CA USA. [Burd, Helcio] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP VanderGheynst, JS (reprint author), Joint BioEnergy Inst, Emeryville, CA USA. EM jsvander@ucdavis.edu RI Thelen, Michael/C-6834-2008; Khudyakov, Jane/C-1213-2014; Thelen, Michael/G-2032-2014; OI Thelen, Michael/0000-0002-2479-5480; Thelen, Michael/0000-0002-2479-5480; Khudyakov, Jane/0000-0001-7038-102X FU University of California Laboratory Fees Research Program [12-LR-237496]; DOE Joint BioEnergy Institute; U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research [DE-AC02-05CH11231]; U.S. Department of Energy FX This work was supported by the University of California Laboratory Fees Research Program #12-LR-237496 and performed as part of the DOE Joint BioEnergy Institute (http://www.jbei.org) supported by the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research, through contract DE-AC02-05CH11231 between Lawrence Berkeley National Laboratory and the U.S. Department of Energy. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 60 TC 12 Z9 12 U1 7 U2 36 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD OCT 25 PY 2013 VL 8 IS 10 AR e77985 DI 10.1371/journal.pone.0077985 PG 12 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 241GW UT WOS:000326155400065 PM 24205054 ER PT J AU Wen, HD Guo, L Barnes, E Lee, JH Walko, DA Schaller, RD Moyer, JA Misra, R Li, YL Dufresne, EM Schlom, DG Gopalan, V Freeland, JW AF Wen, Haidan Guo, Lu Barnes, Eftihia Lee, June Hyuk Walko, Donald A. Schaller, Richard D. Moyer, Jarrett A. Misra, Rajiv Li, Yuelin Dufresne, Eric M. Schlom, Darrell G. Gopalan, Venkatraman Freeland, John W. TI Structural and electronic recovery pathways of a photoexcited ultrathin VO2 film SO PHYSICAL REVIEW B LA English DT Article ID METAL-INSULATOR TRANSITIONS; PHASE-TRANSITION; RUTILE TIO2; EXCITATION; MANGANITE AB The structural and electronic recovery pathways of a photoexcited ultrathin vanadium dioxide (VO2) film at nanosecond time scales have been studied using time-resolved x-ray diffraction and transient optical absorption techniques. The recovery pathways from the tetragonal metallic phase to the monoclinic insulating phase are highly dependent on the optical pump fluence. At pump fluences higher than the saturation fluence of 14.7 mJ/cm(2), we observed a transient structural state with lattice parameter larger than that of the tetragonal phase, which is decoupled from the metal-to-insulator phase transition. Subsequently, the photoexcited VO2 film recovered to the ground state at characteristic times dependent upon the pump fluence as a result of heat transport from the film to the substrate. We present a procedure to measure the time-resolved film temperature by correlating photoexcited and temperature-dependent x-ray diffraction measurements. A thermal transport model that incorporates changes of the thermal parameters across the phase transition reproduces the observed recovery dynamics. The optical excitation and fast recovery of ultrathin VO2 films provides a practical method to reversibly switch between the monoclinic insulating and tetragonal metallic state at nanosecond time scales. C1 [Wen, Haidan; Lee, June Hyuk; Walko, Donald A.; Li, Yuelin; Dufresne, Eric M.; Freeland, John W.] Argonne Natl Lab, Argonne, IL 60439 USA. [Guo, Lu; Barnes, Eftihia; Gopalan, Venkatraman] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. [Schaller, Richard D.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Schaller, Richard D.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Moyer, Jarrett A.] Univ Illinoi Urbana Champaign, Dept Phys, Urbana, IL 61801 USA. [Misra, Rajiv] Penn State Univ, Dept Phys, University Pk, PA 16802 USA. [Schlom, Darrell G.] Cornell Univ, Dept Mat Sci & Engn, Ithaca, NY 14853 USA. [Schlom, Darrell G.] Kavli Inst Cornell Nanoscale Sci, Ithaca, NY 14853 USA. RP Wen, HD (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. EM wen@aps.anl.gov; vxg8@psu.edu; freeland@aps.anl.gov FU US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; Office of Naval Research (ONR) [N00014-11-1-0665] FX Work at Argonne was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. D.G.S. and V.G. would like to acknowledge funding from the Office of Naval Research (ONR) Award No. N00014-11-1-0665. The transport measurements were performed in Peter Schiffer's laboratory. NR 48 TC 14 Z9 14 U1 1 U2 45 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 25 PY 2013 VL 88 IS 16 AR 165424 DI 10.1103/PhysRevB.88.165424 PG 8 WC Physics, Condensed Matter SC Physics GA 240KQ UT WOS:000326095200006 ER PT J AU Ban, CM Xie, M Sun, X Travis, JJ Wang, GK Sun, HT Dillon, AC Lian, J George, SM AF Ban, Chunmei Xie, Ming Sun, Xiang Travis, Jonathan J. Wang, Gongkai Sun, Hongtao Dillon, Anne C. Lian, Jie George, Steven M. TI Atomic layer deposition of amorphous TiO2 on graphene as an anode for Li-ion batteries SO NANOTECHNOLOGY LA English DT Article ID BINARY REACTION SEQUENCE; HIGH AREAL CAPACITY; LITHIUM-STORAGE; ANATASE TIO2; PHOTOCATALYTIC ACTIVITY; CARBON NANOTUBES; THIN-FILMS; OXIDE; GRAPHITE; NANOPARTICLES AB Atomic layer deposition (ALD) was used to deposit TiO2 anode material on high surface area graphene (reduced graphene oxide) sheets for Li-ion batteries. An Al2O3 ALD ultrathin layer was used as an adhesion layer for conformal deposition of the TiO2 ALD films at 120 degrees C onto the conducting graphene sheets. The TiO2 ALD films on the Al2O3 ALD adhesion layer were nearly amorphous and conformal to the graphene sheets. These nanoscale TiO2 coatings minimized the effect of the low diffusion coefficient of lithium ions in bulk TiO2. The TiO2 ALD films exhibited stable capacities of similar to 120 mAh g(-1) and similar to 100 mAh g(-1) at high cycling rates of 1 A g(-1) and 2 A g(-1), respectively. The TiO2 ALD films also displayed excellent cycling stability with similar to 95% of the initial capacity remaining after 500 cycles. These results illustrate that ALD can provide a useful method to deposit electrode materials on high surface area substrates for Li-ion batteries. C1 [Ban, Chunmei; Dillon, Anne C.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Xie, Ming; Travis, Jonathan J.; George, Steven M.] Univ Colorado, Dept Chem & Biochem, Boulder, CO 80309 USA. [Xie, Ming; Travis, Jonathan J.; George, Steven M.] Univ Colorado, Dept Chem & Biol Engn, Boulder, CO 80309 USA. [Sun, Xiang; Wang, Gongkai; Sun, Hongtao; Lian, Jie] Rensselaer Polytech Inst, Dept Mech Aerosp & Nucl Engn, Troy, NY 12180 USA. RP Ban, CM (reprint author), Natl Renewable Energy Lab, 1617 Cole Blvd, Golden, CO 80401 USA. EM ming.xie@colorado.edu; lianj@rpi.edu; steven.george@colorado.edu RI xie, ming/A-1438-2012; Sun, Hongtao/N-6597-2013; George, Steven/O-2163-2013; Wang, Gongkai/A-6504-2015 OI Sun, Hongtao/0000-0003-3259-6091; George, Steven/0000-0003-0253-9184; FU US Department of Energy Office of Vehicle Technologies; Defense Advanced Research Project Agency (DARPA); National Science Foundation [DMR-1151028] FX The research work at National Renewable Energy Laboratory was supported by the US Department of Energy Office of Vehicle Technologies through the Batteries for Advanced Transportation Technologies Program. The work at the University of Colorado was supported by the Defense Advanced Research Project Agency (DARPA). The work at Rensselaer Polytechnic Institute was supported by the National Science Foundation (DMR-1151028). Drs Chunmei Ban and Ming Xie contributed equally to this work. NR 49 TC 35 Z9 35 U1 11 U2 197 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 J9 NANOTECHNOLOGY JI Nanotechnology PD OCT 25 PY 2013 VL 24 IS 42 SI SI AR 424002 DI 10.1088/0957-4484/24/42/424002 PG 6 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA 227VE UT WOS:000325142600004 PM 24067324 ER PT J AU Dunn, B Liu, P Meng, S AF Dunn, Bruce Liu, Ping Meng, Shirley TI Nanoscience and nanotechnology in next generation lithium batteries SO NANOTECHNOLOGY LA English DT Editorial Material C1 [Dunn, Bruce] Univ Calif Los Angeles, Dept Mat Sci & Engn, Los Angeles, CA 90024 USA. [Liu, Ping] US DOE, Adv Res Projects Agcy Energy, Washington, DC 20585 USA. [Meng, Shirley] Univ Calif San Diego, Dept Nanoengn, San Diego, CA 92103 USA. RP Dunn, B (reprint author), Univ Calif Los Angeles, Dept Mat Sci & Engn, Los Angeles, CA 90024 USA. NR 0 TC 3 Z9 3 U1 7 U2 60 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 J9 NANOTECHNOLOGY JI Nanotechnology PD OCT 25 PY 2013 VL 24 IS 42 SI SI AR 420201 DI 10.1088/0957-4484/24/42/420201 PG 1 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA 227VE UT WOS:000325142600001 PM 24195122 ER PT J AU Lee, E Persson, KA AF Lee, Eunseok y Persson, Kristin A. TI First-principles study of the nano-scaling effect on the electrochemical behavior in LiNi0.5Mn1.5O4 SO NANOTECHNOLOGY LA English DT Article ID LI-ION BATTERIES; INITIO MOLECULAR-DYNAMICS; TOTAL-ENERGY CALCULATIONS; JAHN-TELLER DISTORTION; AUGMENTED-WAVE METHOD; THIN-FILM ELECTRODES; CATHODE MATERIALS; CRYSTAL-SURFACES; BASIS-SET; SPINEL AB Nano-scaling of electrode materials is often used in battery applications to enhance performance, particularly relating to rate capability. However, for the high-voltage spinel LiNi0.5Mn1.5O4 conflicting results have been reported on the benefits of nano-scaling. In this study, we present first-principles calculations to investigate the effect of nano-scaling on LiNi0.5Mn1.5O4, specifically focusing on the roles and coupling between surface stability, cation ordering and phase behavior. We calculate and compare the surface energy for the low index facets (100), (110), and (111), and find that the most stable facet is dependent on the cation ordering at the surface layer. In this context, we predict a spontaneous surface reconstruction in the cation-ordered structure which leads to a deviation from the perfect surface cation ordering and results in an enhanced accessibility to solid solution behavior as a function of Li content. Our results imply that nano-scaling will be more beneficial for the cation-ordered structure, as compared to the disordered structure where the solid solution region is already intrinsically accessible for a broad range of Li concentrations. C1 [Lee, Eunseok y; Persson, Kristin A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. RP Lee, E (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. EM eunseoklee@lbl.gov FU Office of Vehicle Technologies of the US Department of Energy [DE-AC02-05CH11231] FX Work at the Lawrence Berkeley National Laboratory was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the US Department of Energy, under Contract No. DE-AC02-05CH11231. We are also grateful to Cheonjoong Kim and Jordi Cabana for enlightening discussions on the high-voltage spinel. NR 40 TC 9 Z9 9 U1 2 U2 75 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 J9 NANOTECHNOLOGY JI Nanotechnology PD OCT 25 PY 2013 VL 24 IS 42 SI SI AR 424007 DI 10.1088/0957-4484/24/42/424007 PG 6 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA 227VE UT WOS:000325142600009 PM 24067535 ER PT J AU Wang, F Wu, LJ Ma, C Su, D Zhu, YM Graetz, J AF Wang, Feng Wu, Lijun Ma, Chao Su, Dong Zhu, Yimei Graetz, Jason TI Excess lithium storage and charge compensation in nanoscale Li4+xTi5O12 SO NANOTECHNOLOGY LA English DT Article ID RECHARGEABLE BATTERIES; CATHODE MATERIALS; SPINEL; LI4TI5O12; INSERTION; NANOPARTICLES; SITES AB Lithium titanate spinel (Li4Ti5O12; LTO) is a promising candidate for anodes in lithium-ion batteries due to its excellent cyclability and safety performance, and has been known as a 'zero-strain' material that allows reversible lithium insertion-deinsertion with little change in the lattice parameters. For a better understanding of lithium reaction mechanisms in this material, it has been of great interest to identify where lithium is inserted and how it migrates during charge and discharge, which is often difficult with x-ray and electron scattering techniques due to the low scattering power of lithium. In this study, we employed atomic-resolution annular bright-field imaging to directly image the lithium on interstitial sites in nanoscale LTO, and electron energy-loss spectroscopy to measure local lithium occupancy and electronic structure at different states of charge. During lithiation, charge compensation occurs primarily at O sites, rather than at Ti sites, and no significant change was found in the projected density of states (Ti 3d) until the voltage was lowered to similar to 50 mV or below. The Li K-edge spectra were simulated via ab initio calculations, providing a direct correlation between the near-edge fine structure and the local lithium coordination. During the initial states of discharge, lithium ions on 8a sites migrate to 16c sites (above 740 mV). Further lithiation causes the partial re-occupation of 8a sites, initially in the near-surface region at similar to 600 mV, and then in the bulk at lower voltages (similar to 50 mV). We attribute the enhanced capacity in nanostructured LTO to extra storage of lithium in the near-surface region, primarily at {111} facets. C1 [Wang, Feng; Wu, Lijun; Ma, Chao; Su, Dong; Zhu, Yimei; Graetz, Jason] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Wang, F (reprint author), Brookhaven Natl Lab, Upton, NY 11973 USA. EM fwang@bnl.gov RI Ma, Chao/J-4569-2015; Wang, Feng/C-1443-2016; Su, Dong/A-8233-2013 OI Wang, Feng/0000-0003-4068-9212; Su, Dong/0000-0002-1921-6683 FU New York Battery and Energy Storage Technology (NY-BEST) Consortium [18509]; US DOE, Office of Science [DE-AC02-98CH10886] FX This work was partially supported by New York Battery and Energy Storage Technology (NY-BEST) Consortium, under Contract No. 18509. We thank Ganesh Venugopal and Andrew Hunt from nGimat for providing the Li4Ti5O12 samples. We thank Jian Hong, Joseph Woicik, and Daniel Fisher for help with sample processing and synchrotron XPS measurements. XPS measurement at the National Synchrotron Light Source, Brookhaven National Laboratory, was supported by the US DOE, Office of Science, under Contract No. DE-AC02-98CH10886. NR 31 TC 6 Z9 6 U1 2 U2 67 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 J9 NANOTECHNOLOGY JI Nanotechnology PD OCT 25 PY 2013 VL 24 IS 42 SI SI AR 424006 DI 10.1088/0957-4484/24/42/424006 PG 8 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA 227VE UT WOS:000325142600008 PM 24067496 ER PT J AU Wu, J Dathar, GKP Sun, CW Theivanayagam, MG Applestone, D Dylla, AG Manthiram, A Henkelman, G Goodenough, JB Stevenson, KJ AF Wu, Jing Dathar, Gopi Krishna Phani Sun, Chunwen Theivanayagam, Murali G. Applestone, Danielle Dylla, Anthony G. Manthiram, Arumugam Henkelman, Graeme Goodenough, John B. Stevenson, Keith J. TI In situ Raman spectroscopy of LiFePO4: size and morphology dependence during charge and self-discharge SO NANOTECHNOLOGY LA English DT Article ID TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; LI-INSERTION/EXTRACTION; PARTICLE-SIZE; BATTERIES; ELECTRODES; LIXFEPO4; CATHODES AB Previous studies of the size dependent properties of LiFePO4 have focused on the diffusion rate or phase transformation pathways by bulk analysis techniques such as x-ray diffraction (XRD), neutron diffraction and electrochemistry. In this work, in situ Raman spectroscopy was used to study the surface phase change during charge and self-discharge on a more localized scale for three morphologies of LiFePO4: (1) 25 +/- 6 nm width nanorods, (2) 25 +/- 6 nm width nanorods and (3) similar to 2 mu m porous microspheres. Both the large nanorod and microsphere geometries showed incomplete delithiation at the end of charge, which was most likely caused by anti-site defects along the 1D diffusion channels in the bulk of the larger particles. Based on the in situ Raman measurements, all of the morphologies studied exhibited self-discharge with time. Among them, the smallest FePO4 particles self-discharged (lithiated) the fastest. While nanostructuring LiFePO4 can offer advantages in terms of lowering anti-site defects within particles, it also creates new problems due to high surface energies that allow self-discharge. The in situ Raman spectroscopy also showed that carbon coating did not provide significant improvement to the stability of the lithiated particles. C1 [Wu, Jing; Dylla, Anthony G.; Henkelman, Graeme; Stevenson, Keith J.] Univ Texas Austin, Dept Chem & Biochem, Austin, TX 78712 USA. [Dathar, Gopi Krishna Phani] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN USA. [Sun, Chunwen] Chinese Acad Sci, Inst Phys, Beijing 100080, Peoples R China. [Theivanayagam, Murali G.; Manthiram, Arumugam] Univ Texas Austin, Texas Mat Inst, Austin, TX 78712 USA. [Applestone, Danielle] Otherlab Inc, San Francisco, CA USA. [Goodenough, John B.] Univ Texas Austin, Mat Sci & Engn Program, Austin, TX 78712 USA. RP Stevenson, KJ (reprint author), Univ Texas Austin, Dept Chem & Biochem, Austin, TX 78712 USA. EM stevenson@cm.utexas.edu RI Sun, Chunwen/A-9860-2008 OI Sun, Chunwen/0000-0002-3610-9396 FU US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001091]; Office of Science of the US Department of Energy [DE-AC02-05CH11231]; program 'Understanding Charge Separation and Transfer at Interfaces in Energy Materials (EFRC:CST)'; Energy Frontier Research Center FX This material is based upon work supported as part of the program 'Understanding Charge Separation and Transfer at Interfaces in Energy Materials (EFRC:CST)', an Energy Frontier Research Center funded by the US Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number DE-SC0001091. We also acknowledge the computational resources from National Energy Research Scientific Computing Center (NERSC), which is supported by the Office of Science of the US Department of Energy under Contract No. DE-AC02-05CH11231. NR 26 TC 10 Z9 12 U1 10 U2 106 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 J9 NANOTECHNOLOGY JI Nanotechnology PD OCT 25 PY 2013 VL 24 IS 42 SI SI AR 424009 DI 10.1088/0957-4484/24/42/424009 PG 9 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA 227VE UT WOS:000325142600011 PM 24067625 ER PT J AU Xiao, J Zheng, JM Li, XL Shao, YY Zhang, JG AF Xiao, Jie Zheng, Jianming Li, Xiaolin Shao, Yuyan Zhang, Ji-Guang TI Hierarchically structured materials for lithium batteries SO NANOTECHNOLOGY LA English DT Article ID RECHARGEABLE LI-O-2 BATTERIES; LI-AIR BATTERIES; ION BATTERIES; CATHODE MATERIALS; OXYGEN REDUCTION; OXIDE COMPOSITE; POROUS CARBON; SILICON ANODE; LONG-LIFE; ELECTRODES AB The lithium-ion battery (LIB) is one of the most promising power sources to be deployed in electric vehicles, including solely battery powered vehicles, plug-in hybrid electric vehicles, and hybrid electric vehicles. With the increasing demand for devices of high-energy densities (> 500 Wh kg(-1)), new energy storage systems, such as lithium-oxygen (Li-O-2) batteries and other emerging systems beyond the conventional LIB, have attracted worldwide interest for both transportation and grid energy storage applications in recent years. It is well known that the electrochemical performance of these energy storage systems depends not only on the composition of the materials, but also on the structure of the electrode materials used in the batteries. Although the desired performance characteristics of batteries often have conflicting requirements with the micro/nano-structure of electrodes, hierarchically designed electrodes can be tailored to satisfy these conflicting requirements. This work will review hierarchically structured materials that have been successfully used in LIB and Li-O-2 batteries. Our goal is to elucidate (1) how to realize the full potential of energy materials through the manipulation of morphologies, and (2) how the hierarchical structure benefits the charge transport, promotes the interfacial properties and prolongs the electrode stability and battery lifetime. C1 [Xiao, Jie; Zheng, Jianming; Li, Xiaolin; Shao, Yuyan; Zhang, Ji-Guang] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. RP Xiao, J (reprint author), Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. EM jiguang.zhang@pnnl.gov RI Shao, Yuyan/A-9911-2008; Zheng, Jianming/F-2517-2014 OI Shao, Yuyan/0000-0001-5735-2670; Zheng, Jianming/0000-0002-4928-8194 FU US Department of Energy's Office of Energy Efficiency and Renewable Energy, Office of Vehicle Technologies FX We gratefully acknowledge the support provided by the US Department of Energy's Office of Energy Efficiency and Renewable Energy, Office of Vehicle Technologies. NR 48 TC 14 Z9 14 U1 8 U2 131 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 EI 1361-6528 J9 NANOTECHNOLOGY JI Nanotechnology PD OCT 25 PY 2013 VL 24 IS 42 SI SI AR 424004 DI 10.1088/0957-4484/24/42/424004 PG 7 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA 227VE UT WOS:000325142600006 PM 24067410 ER PT J AU Attanasio, C Nord, AS Zhu, YW Blow, MJ Li, ZR Liberton, DK Morrison, H Plajzer-Frick, I Holt, A Hosseini, R Phouanenavong, S Akiyama, JA Shoukry, M Afzal, V Rubin, EM FitzPatrick, DR Ren, B Hallgrimsson, B Pennacchio, LA Visel, A AF Attanasio, Catia Nord, Alex S. Zhu, Yiwen Blow, Matthew J. Li, Zirong Liberton, Denise K. Morrison, Harris Plajzer-Frick, Ingrid Holt, Amy Hosseini, Roya Phouanenavong, Sengthavy Akiyama, Jennifer A. Shoukry, Malak Afzal, Veena Rubin, Edward M. FitzPatrick, David R. Ren, Bing Hallgrimsson, Benedikt Pennacchio, Len A. Visel, Axel TI Fine Tuning of Craniofacial Morphology by Distant-Acting Enhancers SO SCIENCE LA English DT Article ID GENOME-WIDE ASSOCIATION; CLEFT-LIP; GENE-EXPRESSION; NEURAL CREST; TOOTH DEVELOPMENT; SONIC HEDGEHOG; CRANIAL BASE; PALATE; MOUSE; MICE AB The shape of the human face and skull is largely genetically determined. However, the genomic basis of craniofacial morphology is incompletely understood and hypothesized to involve protein-coding genes, as well as gene regulatory sequences. We used a combination of epigenomic profiling, in vivo characterization of candidate enhancer sequences in transgenic mice, and targeted deletion experiments to examine the role of distant-acting enhancers in craniofacial development. We identified complex regulatory landscapes consisting of enhancers that drive spatially complex developmental expression patterns. Analysis of mouse lines in which individual craniofacial enhancers had been deleted revealed significant alterations of craniofacial shape, demonstrating the functional importance of enhancers in defining face and skull morphology. These results demonstrate that enhancers are involved in craniofacial development and suggest that enhancer sequence variation contributes to the diversity of human facial morphology. C1 [Attanasio, Catia; Nord, Alex S.; Zhu, Yiwen; Plajzer-Frick, Ingrid; Holt, Amy; Hosseini, Roya; Phouanenavong, Sengthavy; Akiyama, Jennifer A.; Shoukry, Malak; Afzal, Veena; Rubin, Edward M.; Pennacchio, Len A.; Visel, Axel] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Blow, Matthew J.; Rubin, Edward M.; Pennacchio, Len A.; Visel, Axel] US DOE, Joint Genome Inst, Walnut Creek, CA 94598 USA. [Li, Zirong; Ren, Bing] Univ Calif San Diego, Sch Med, Ludwig Inst Canc Res, La Jolla, CA 92093 USA. [Li, Zirong; Ren, Bing] Univ Calif San Diego, Sch Med, Dept Cellular & Mol Med, La Jolla, CA 92093 USA. [Liberton, Denise K.; Hallgrimsson, Benedikt] Univ Calgary, Dept Cell Biol & Anat, McCaig Bone & Joint Inst, Calgary, AB T2N 4N1, Canada. [Morrison, Harris; FitzPatrick, David R.] Univ Edinburgh, MRC Inst Genet & Mol Med, MRC Human Genet Unit, Edinburgh EH4 2XU, Midlothian, Scotland. [FitzPatrick, David R.] Royal Hosp Sick Children, Edinburgh EH9 1LF, Midlothian, Scotland. [Hallgrimsson, Benedikt] Univ Calgary, Alberta Childrens Hosp, Res Inst, Calgary, AB T2N 4N1, Canada. RP Visel, A (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM avisel@lbl.gov RI Visel, Axel/A-9398-2009; Blow, Matthew/G-6369-2012; attanasio, catia/D-5042-2017; Hallgrimsson, Benedikt/A-9616-2008; OI Visel, Axel/0000-0002-4130-7784; Blow, Matthew/0000-0002-8844-9149; Hallgrimsson, Benedikt/0000-0002-7192-9103; FitzPatrick, David R./0000-0003-4861-969X FU NIDCR FaceBase grant [U01DE020060]; National Human Genome Research Institute [R01HG003988, U54HG006997]; Swiss National Science Foundation; F32 NIH/National Institute of General Medical Sciences National Research Service Award [GM105202]; NIH [U54HG006997, 1R01DE021708, 1R01DE01963, 1U01DE020054, R01HG003991]; Natural Sciences and Engineering Research Council of Canada [238992-11]; UK Medical Research Council; Ludwig Institute for Cancer Research; NIH; Department of Energy [DE-AC02-05CH11231] FX The authors thank J. Harkes and M. Satyanarayanan for development of the OPT viewer; S. Shen and H. Hochheiser for integration of the OPT viewer and data sets into FaceBase; and J. Murray, M. Marazita, J. Manak, B. Schutte, and all FaceBase members for help in the selection of relevant craniofacial intervals and comments on results. A. V. and L. A. P. were supported by NIDCR FaceBase grant U01DE020060 and by National Human Genome Research Institute grants R01HG003988 and U54HG006997. C. A. was supported by a Swiss National Science Foundation advanced researcher fellowship. A. S. N. was supported by a F32 NIH/National Institute of General Medical Sciences National Research Service Award fellowship GM105202. B. H. was supported by NIH 1R01DE021708, NIH 1R01DE01963, NIH 1U01DE020054, and Natural Sciences and Engineering Research Council of Canada #238992-11 grants. D. R. F. and H. M. were supported by a UK Medical Research Council core program grant. B. R. was supported by the Ludwig Institute for Cancer Research and NIH grants U54HG006997 and R01HG003991. B. H. was supported by NIH 1R01DE01963. Research was conducted at the E. O. Lawrence Berkeley National Laboratory and performed under Department of Energy contract DE-AC02-05CH11231, University of California. ChIP-Seq data are available through GEO (accession no. GSE49413) and FaceBase. org. In vivo reporter data are available through the Vista Enhancer Browser (http://enhancer.lbl.gov) and FaceBase. org. OPT data, including raw images and interactive 3D viewing option, is available through http://facebase.org. All enhancer reporter vectors, as well as archived surplus LacZ-stained embryos for selected enhancers, are available from the authors. Craniofacial enhancer knockout lines are available through the Mutant Mouse Regional Resource Centers (Delta hs1431, MMRRC 03895; Delta hs746, MMRRC 03888; and Delta hs586, MMRRCC 03894). NR 61 TC 77 Z9 79 U1 3 U2 20 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD OCT 25 PY 2013 VL 342 IS 6157 AR 1241006 DI 10.1126/science.1241006 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 239RH UT WOS:000326042600032 PM 24159046 ER PT J AU Rocha, C Calado, R Borrego, P Marcelino, JM Bartolo, I Rosado, L Cavaco-Silva, P Gomes, P Familia, C Quintas, A Skar, H Leitner, T Barroso, H Taveira, N AF Rocha, Cheila Calado, Rita Borrego, Pedro Marcelino, Jose Maria Bartolo, Ines Rosado, Lino Cavaco-Silva, Patricia Gomes, Perpetua Familia, Carlos Quintas, Alexandre Skar, Helena Leitner, Thomas Barroso, Helena Taveira, Nuno TI Evolution of the human immunodeficiency virus type 2 envelope in the first years of infection is associated with the dynamics of the neutralizing antibody response SO RETROVIROLOGY LA English DT Article DE Vertical HIV-2 infection; Evolution of the neutralizing antibody response; Escape from neutralization; Molecular evolution; Tropism ID PLASMA VIRAL LOAD; HIV-2 INFECTION; GUINEA-BISSAU; VERTICAL TRANSMISSION; PHYLOGENETIC ANALYSIS; CLINICAL PROGRESSION; CORECEPTOR USAGE; SWISS-MODEL; WEST-AFRICA; V3 LOOP AB Background: Differently from HIV-1, HIV-2 disease progression usually takes decades without antiretroviral therapy and the majority of HIV-2 infected individuals survive as elite controllers with normal CD4(+) T cell counts and low or undetectable plasma viral load. Neutralizing antibodies (Nabs) are thought to play a central role in HIV-2 evolution and pathogenesis. However, the dynamic of the Nab response and resulting HIV-2 escape during acute infection and their impact in HIV-2 evolution and disease progression remain largely unknown. Our objective was to characterize the Nab response and the molecular and phenotypic evolution of HIV-2 in association with Nab escape in the first years of infection in two children infected at birth. Results: CD4+ T cells decreased from about 50% to below 30% in both children in the first five years of infection and the infecting R5 viruses were replaced by X4 viruses within the same period. With antiretroviral therapy, viral load in child 1 decreased to undetectable levels and CD4(+) T cells recovered to normal levels, which have been sustained at least until the age of 12. In contrast, viral load increased in child 2 and she progressed to AIDS and death at age 9. Beginning in the first year of life, child 1 raised high titers of antibodies that neutralized primary R5 isolates more effectively than X4 isolates, both autologous and heterologous. Child 2 raised a weak X4-specific Nab response that decreased sharply as disease progressed. Rate of evolution, nucleotide and amino acid diversity, and positive selection, were significantly higher in the envelope of child 1 compared to child 2. Rates of R5-to-X4 tropism switch, of V1 and V3 sequence diversification, and of convergence of V3 to a beta-hairpin structure were related with rate of escape from the neutralizing antibodies. Conclusion: Our data suggests that the molecular and phenotypic evolution of the human immunodeficiency virus type 2 envelope are related with the dynamics of the neutralizing antibody response providing further support for a model in which Nabs play an important role in HIV-2 pathogenesis. C1 [Rocha, Cheila; Calado, Rita; Borrego, Pedro; Bartolo, Ines; Barroso, Helena; Taveira, Nuno] Fac Farm Lisboa, Ctr Patogenese Mol, Unidade Retrovirus Infeccoes Assoc, Lisbon, Portugal. [Rocha, Cheila; Calado, Rita; Borrego, Pedro; Bartolo, Ines; Cavaco-Silva, Patricia; Gomes, Perpetua; Familia, Carlos; Quintas, Alexandre; Barroso, Helena; Taveira, Nuno] Inst Super Ciencias Saude Egas Moniz, Ctr Invest Interdisciplinar Egas Moniz CiiEM, Monte De Caparica, Portugal. [Marcelino, Jose Maria] Univ Nova Lisboa, Inst Higiene & Med Trop, Unidade Microbiol Med, P-1200 Lisbon, Portugal. [Rosado, Lino] Hosp Dona Estefania, Unidade Imunohematol, Lisbon, Portugal. [Gomes, Perpetua] Ctr Hosp Lisboa Ocidental HEM, Serv Med Transfus, Lab Biol Mol, Lisbon, Portugal. [Gomes, Perpetua] Inst Super Higiene & Med Trop, Ctr Malaria & Outras Doencas Tropicais, Lisbon, Portugal. [Skar, Helena; Leitner, Thomas] Los Alamos Natl Lab, Los Alamos, NM USA. RP Taveira, N (reprint author), Fac Farm Lisboa, Ctr Patogenese Mol, Unidade Retrovirus Infeccoes Assoc, Lisbon, Portugal. EM ntaveira@ff.ul.pt RI iMed.ULisboa, EEPHIV /B-4222-2014; iMed.ULisboa, iMed.ULisboa/C-6292-2014; Bartolo, Ines/A-7477-2014; Rocha, Cheila/E-8776-2015; Gomes, Perpetua/I-5652-2012; Marcelino, Jose Maria/B-3374-2008; Familia, Carlos/A-4535-2013; Borrego, Pedro/H-6968-2013; Taveira, Nuno/A-6252-2014; Quintas, Alexandre/J-6436-2012 OI Barroso, Helena/0000-0003-4098-5433; Bartolo, Ines/0000-0002-2022-8921; Rocha, Cheila/0000-0002-0148-9405; Gomes, Perpetua/0000-0003-3271-8255; Montez, Patricia/0000-0002-2463-0176; Marcelino, Jose Maria/0000-0002-4597-1535; Familia, Carlos/0000-0001-5059-2487; Borrego, Pedro/0000-0002-1949-9484; Taveira, Nuno/0000-0003-0176-5585; Quintas, Alexandre/0000-0002-5188-0453 FU Fundacao para a Ciencia e Tecnologia (FCT), Portugal [PTDC/SAU-FAR/115290/2009, PTDC/SAU-EPI/122400/2010]; NIH [R01AI087520]; Collaborative HIV and Anti-HIV Drug Resistance Network (CHAIN); European Union; Fundacao para a Ciencia e Tecnologia, Portugal; Swedish Research Council [623-2011-1100] FX This work was supported by grants PTDC/SAU-FAR/115290/2009 and PTDC/SAU-EPI/122400/2010 from Fundacao para a Ciencia e Tecnologia (FCT) (http://www.fct.pt), Portugal, a NIH grant (R01AI087520), and by Collaborative HIV and Anti-HIV Drug Resistance Network (CHAIN), from the European Union. Cheila Rocha, Rita Calado, Pedro Borrego and Ines Bartolo were supported by PhD scholarships from Fundacao para a Ciencia e Tecnologia, Portugal. Helena Skar was supported by a postdoctoral fellowship from the Swedish Research Council (623-2011-1100). The following reagents were obtained through the AIDS Research and Reference Reagent Program, NR 74 TC 3 Z9 3 U1 2 U2 8 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1742-4690 J9 RETROVIROLOGY JI Retrovirology PD OCT 24 PY 2013 VL 10 AR 110 DI 10.1186/1742-4690-10-110 PG 14 WC Virology SC Virology GA 280PP UT WOS:000329043500002 PM 24156513 ER PT J AU Barouch, DH Stephenson, KE Borducchi, EN Smith, K Stanley, K McNally, AG Liu, JY Abbink, P Maxfield, LF Seaman, MS Dugast, AS Alter, G Ferguson, M Li, WJ Earl, PL Moss, B Giorgi, EE Szinger, JJ Eller, LA Billings, EA Rao, M Tovanabutra, S Sanders-Buell, E Weijtens, M Pau, MG Schuitemaker, H Robb, ML Kim, JH Korber, BT Michael, NL AF Barouch, Dan H. Stephenson, Kathryn E. Borducchi, Erica N. Smith, Kaitlin Stanley, Kelly McNally, Anna G. Liu, Jinyan Abbink, Peter Maxfield, Lori F. Seaman, Michael S. Dugast, Anne-Sophie Alter, Galit Ferguson, Melissa Li, Wenjun Earl, Patricia L. Moss, Bernard Giorgi, Elena E. Szinger, James J. Eller, Leigh Anne Billings, Erik A. Rao, Mangala Tovanabutra, Sodsai Sanders-Buell, Eric Weijtens, Mo Pau, Maria G. Schuitemaker, Hanneke Robb, Merlin L. Kim, Jerome H. Korber, Bette T. Michael, Nelson L. TI Protective Efficacy of a Global HIV-1 Mosaic Vaccine against Heterologous SHIV Challenges in Rhesus Monkeys SO CELL LA English DT Article ID SIMIAN IMMUNODEFICIENCY VIRUS; T-LYMPHOCYTE RESPONSES; NEUTRALIZING ANTIBODIES; IMMUNE CONTROL; REPLICATION; DIVERSITY; MACAQUES; BREADTH; AIDS; IMMUNOGENICITY AB The global diversity of HIV-1 represents a critical challenge facing HIV-1 vaccine development. HIV-1 mosaic antigens are bioinformatically optimized immunogens designed for improved coverage of HIV-1 diversity. However, the protective efficacy of such global HIV-1 vaccine antigens has not previously been evaluated. Here, we demonstrate the capacity of bivalent HIV-1 mosaic antigens to protect rhesus monkeys against acquisition of infection following heterologous challenges with the difficult-to-neutralize simian-human immunodeficiency virus SHIV-SF162P3. Adenovirus/poxvirus and adenovirus/adenovirus vector-based vaccines expressing HIV-1 mosaic Env, Gag, and Pol afforded a significant reduction in the per-exposure acquisition risk following repetitive, intrarectal SHIV-SF162P3 challenges. Protection against acquisition of infection correlated with vaccine-elicited binding, neutralizing, and functional nonneutralizing antibodies, suggesting that the coordinated activity of multiple antibody functions may contribute to protection against difficult-to-neutralize viruses. These data demonstrate the protective efficacy of HIV-1 mosaic antigens and suggest a potential strategy for the development of a global HIV-1 vaccine. C1 [Barouch, Dan H.; Stephenson, Kathryn E.; Borducchi, Erica N.; Smith, Kaitlin; Stanley, Kelly; McNally, Anna G.; Liu, Jinyan; Abbink, Peter; Maxfield, Lori F.; Seaman, Michael S.] Harvard Univ, Beth Israel Deaconess Med Ctr, Sch Med, Ctr Virol & Vaccine Res, Boston, MA 02215 USA. [Barouch, Dan H.; Dugast, Anne-Sophie; Alter, Galit] Ragon Inst MGH Massachusetts Inst Technol & Harva, Boston, MA 02114 USA. [Ferguson, Melissa] Alpha Genesis Inc, Yemassee, SC 29945 USA. [Li, Wenjun] Univ Massachusetts, Sch Med, Worcester, MA 01605 USA. [Earl, Patricia L.; Moss, Bernard] NIAID, Bethesda, MD 20892 USA. [Giorgi, Elena E.; Szinger, James J.; Korber, Bette T.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Eller, Leigh Anne; Billings, Erik A.; Rao, Mangala; Tovanabutra, Sodsai; Sanders-Buell, Eric; Robb, Merlin L.; Kim, Jerome H.; Michael, Nelson L.] Walter Reed Army Inst Res, US Mil HIV Res Program, Rockville, MD 20850 USA. [Weijtens, Mo; Pau, Maria G.; Schuitemaker, Hanneke] Crucell Holland BV, NL-2301 CA Leiden, Netherlands. RP Barouch, DH (reprint author), Harvard Univ, Beth Israel Deaconess Med Ctr, Sch Med, Ctr Virol & Vaccine Res, Boston, MA 02215 USA. EM dbarouch@bidmc.harvard.edu RI Li, Wenjun/F-5634-2015; Dugast, AnneSophie/L-9541-2015 OI Li, Wenjun/0000-0001-5335-7386; FU U.S. Military Research and Material Command; U.S. Military HIV Research Program [W81XWH-07-2-0067]; National Institutes of Health [AI052074, AI060354, AI078526, AI084794, AI095985, AI096040, AI100645]; NIAID Division of Intramural Research; Ragon Institute of MGH, MIT, and Harvard; Bill and Melinda Gates Foundation [OPP1033091, OPP1040741] FX We thank M. Pensiero, S. Blackmore, R. Bradsky, C. Cabral, A. Cheung, J. Goudsmit, R. Hamel, B. Hibl, S. Howell, M. Iampietro, K. Kelly, D. Lynch, M. Marovich, C. Miller, J. Nkolola, A. O'Sullivan, L. Parenteau, J. Perry, W. Rinaldi, J. Sadoff, A. SanMiguel, N. Simmons, J. Smith, F. Stephens, D. van Manen, G. Westergaard, and L. Wyatt for generous advice, assistance, and reagents. The HIV-1 PTE peptides were obtained from the NIH AIDS Research and Reference Reagent Program. We acknowledge support from the U.S. Military Research and Material Command and the U.S. Military HIV Research Program (W81XWH-07-2-0067); the National Institutes of Health (AI052074, AI060354, AI078526, AI084794, AI095985, AI096040, and AI100645); the NIAID Division of Intramural Research; the Ragon Institute of MGH, MIT, and Harvard; and the Bill and Melinda Gates Foundation (OPP1033091 and OPP1040741). M. W., M. G. P., and H. S. are employees of Crucell. Beth Israel Deaconess Medical Center and Los Alamos National Laboratory are co-owners of an HIV-1 mosaic antigen patent that has been licensed to Crucell. The opinions in this manuscript are those of the authors and do not reflect the views of the U.S. Department of the Army or the Department of Defense. NR 37 TC 103 Z9 103 U1 1 U2 12 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0092-8674 EI 1097-4172 J9 CELL JI Cell PD OCT 24 PY 2013 VL 155 IS 3 BP 531 EP 539 DI 10.1016/j.cell.2013.09.061 PG 9 WC Biochemistry & Molecular Biology; Cell Biology SC Biochemistry & Molecular Biology; Cell Biology GA 246WQ UT WOS:000326571800009 PM 24243013 ER PT J AU Fang, XY Wang, JB O'Carroll, IP Mitchell, M Zuo, XB Wang, Y Yu, P Liu, Y Rausch, JW Dyba, MA Kjems, J Schwieters, CD Seifert, S Winans, RE Watts, NR Stahl, SJ Wingfield, PT Byrd, RA Le Grice, SFJ Rein, A Wang, YX AF Fang, Xianyang Wang, Jinbu O'Carroll, Ina P. Mitchell, Michelle Zuo, Xiaobing Wang, Yi Yu, Ping Liu, Yu Rausch, Jason W. Dyba, Marzena A. Kjems, Jorgen Schwieters, Charles D. Seifert, Soenke Winans, Randall E. Watts, Norman R. Stahl, Stephen J. Wingfield, Paul T. Byrd, R. Andrew Le Grice, Stuart F. J. Rein, Alan Wang, Yun-Xing TI An Unusual Topological Structure of the HIV-1 Rev Response Element SO CELL LA English DT Article ID SMALL-ANGLE SCATTERING; X-RAY-SCATTERING; GENE-EXPRESSION REQUIRES; RICH-BINDING MOTIF; BIOLOGICAL MACROMOLECULES; SECONDARY STRUCTURE; ZINC-FINGER; VIRION EXPRESSION; TRANS-ACTIVATOR; TARGET SEQUENCE AB Nuclear export of unspliced and singly spliced viral mRNA is a critical step in the HIV life cycle. The structural basis by which the virus selects its own mRNA among more abundant host cellular RNAs for export has been a mystery for more than 25 years. Here, we describe an unusual topological structure that the virus uses to recognize its own mRNA. The viral Rev response element (RRE) adopts an "A"-like structure in which the two legs constitute two tracks of binding sites for the viral Rev protein and position the two primary known Rev-binding sites similar to 55 angstrom apart, matching the distance between the two RNAbinding motifs in the Rev dimer. Both the legs of the "A" and the separation between them are required for optimal RRE function. This structure accounts for the specificity of Rev for the RRE and thus the specific recognition of the viral RNA. C1 [Fang, Xianyang; Wang, Jinbu; Zuo, Xiaobing; Yu, Ping; Liu, Yu; Wang, Yun-Xing] NCI, Prot Nucle Acid Interact Sect, Struct Biophys Lab, HIV Drug Resistance Program,Ctr Canc Res,NIH, Frederick, MD 21702 USA. [O'Carroll, Ina P.; Rein, Alan] NCI, Retroviral Assembly Sect, HIV Drug Resistance Program, Ctr Canc Res,NIH, Frederick, MD 21702 USA. [Mitchell, Michelle; Wang, Yi; Rausch, Jason W.; Le Grice, Stuart F. J.] NCI, RT Biochem Sect, HIV Drug Resistance Program, Ctr Canc Res,NIH, Frederick, MD 21702 USA. [Yu, Ping; Dyba, Marzena A.] SAIC Frederick, Struct Biophys Lab, Frederick, MD 21702 USA. [Kjems, Jorgen] Univ Aarhus, Dept Mol Biol, DK-8000 Aarhus C, Denmark. [Schwieters, Charles D.] NIH, Div Computat Biosci, Ctr Informat Technol, Bethesda, MD 20892 USA. [Seifert, Soenke; Winans, Randall E.] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. [Watts, Norman R.; Stahl, Stephen J.; Wingfield, Paul T.] NIAMSD, Prot Express Lab, NIH, Bethesda, MD 20892 USA. [Byrd, R. Andrew] NCI, Macromol NMR Sect, Struct Biophys Lab, Ctr Canc Res,NIH, Frederick, MD 21702 USA. RP Rein, A (reprint author), NCI, Retroviral Assembly Sect, HIV Drug Resistance Program, Ctr Canc Res,NIH, Frederick, MD 21702 USA. EM reina@mail.nih.gov; wangyunx@mail.nih.gov RI Byrd, R. Andrew/F-8042-2015 OI Byrd, R. Andrew/0000-0003-3625-4232 FU Intramural Research Program of the National Institutes of Health, National Cancer Institute (NCI) Center for Cancer Research; National Institute of Arthritis, Musculoskeletal and Skin Diseases; Center for Information Technology; SAIC-Frederick [HHSN26120080001E]; U.S. DOE [DE-AC02-06CH11357] FX We thank Drs. Stephen Hughes, Alexander Wlodawer, and Prof. James Williamson for discussion. This work was supported in part by the Intramural Research Program of the National Institutes of Health, National Cancer Institute (NCI) Center for Cancer Research; National Institute of Arthritis, Musculoskeletal and Skin Diseases; Center for Information Technology; and SAIC-Frederick under contract HHSN26120080001E. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. The content of this publication does not necessarily reflect the views or policies of the Department of Health and Human Services, nor does mention of trade names, commercial products or organizations imply endorsement by the US Government. NR 57 TC 52 Z9 52 U1 3 U2 25 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0092-8674 EI 1097-4172 J9 CELL JI Cell PD OCT 24 PY 2013 VL 155 IS 3 BP 594 EP 605 DI 10.1016/j.cell.2013.10.008 PG 12 WC Biochemistry & Molecular Biology; Cell Biology SC Biochemistry & Molecular Biology; Cell Biology GA 246WQ UT WOS:000326571800014 PM 24243017 ER PT J AU Zhao, J Scheibe, TD Mahadevan, R AF Zhao, Jiao Scheibe, T. D. Mahadevan, R. TI Model-based analysis of mixed uranium(VI) reduction by biotic and abiotic pathways during in situ bioremediation SO CHEMICAL GEOLOGY LA English DT Article DE Abiotic pathways; Biotic pathways; Field conditions; Mixed U(VI) reduction; Mackinawite ID SULFATE-REDUCING BACTERIA; MICROBIAL REDUCTION; CONTAMINATED AQUIFER; IRON(II); FE(III); U(VI); GROUNDWATER; SEDIMENTS; DYNAMICS; OXIDES AB Given the numerous unknowns and uncertainties in sediment systems, understanding of the mechanisms of U(VI) reduction is still at the stage of improvement. Recent studies have shown that reductive immobilization of U(VI) in the subsurface is not caused by purely biological or purely abiotic reactions but rather a group of interconnected abiotic-biotic pathways (e. g. via mackinawite and biomass). These new findings necessitate an update of the existing mathematical models that make simplifications typically involving a single reducing agent (e. g. indigenous bacteria) for in situ bioremediation of uranium-contaminated groundwater. In this study, a comprehensive model was constructed based on new experimental observations, including mixed U(VI) reduction by chemical and enzymatic reactions. Thermodynamic analysis was done to predict the feasibility of the potential pathways that affect mackinawite formation under field conditions. Model simulations indicate that low concentrations of the reactant species make the reaction of homogeneous Fe(II) oxidation coupled to U(VI) reduction unfavorable in the field. Instead, FeS precipitation is an important Fe(II) sequestration reaction once sulfate metabolism dominates. The subsequent reduction of U(VI) by FeS (mackinawite) contributes to the total U(VI) removal under a variety of U(VI) concentrations encountered at field sites, which is in accordance with experimental observations. The model suggests the potential for both competition and coordination between chemical and biological pathways on the cell surface, providing a possible explanation as to why U(VI) can be efficiently reduced at either low or high sulfate concentration during the process of in situ bioremediation. Further increase in the resolution of the model (e. g. across multiple scales such as genome-, micron- and pore-sale) is necessary for better understanding of the interactions between biotic and abiotic pathways. (C) 2013 Elsevier B.V. All rights reserved. C1 [Zhao, Jiao; Mahadevan, R.] Univ Toronto, Dept Chem Engn & Appl Chem, Biozone, Toronto, ON M5S 3E5, Canada. [Mahadevan, R.] Univ Toronto, Inst Biomat & Biomed Engn, Toronto, ON M5S 3G9, Canada. [Scheibe, T. D.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Zhao, J (reprint author), Univ Toronto, Dept Chem Engn & Appl Chem, 200 Coll St, Toronto, ON M5S 3E5, Canada. EM jiao.zhao@utoronto.ca RI Scheibe, Timothy/A-8788-2008; Mahadevan, Radhakrishnan/A-8502-2008 OI Scheibe, Timothy/0000-0002-8864-5772; Mahadevan, Radhakrishnan/0000-0002-1270-9063 FU Office of Science (BER), U.S. Department of Energy [DE-FG02-07ER64367, DE-FC02-02ER63446]; Office of Science (BER), U.S. Department of Energy from the Environmental Remediation Sciences Program FX This research was supported by the Office of Science (BER), U.S. Department of Energy from grant DE-FG02-07ER64367 from the Environmental Remediation Sciences Program and Cooperative Agreement DE-FC02-02ER63446. The Sun Grid Infrastructure was provided by Compute Canada National Resource Allocation Award 2011-2013. NR 35 TC 2 Z9 2 U1 4 U2 24 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2541 EI 1878-5999 J9 CHEM GEOL JI Chem. Geol. PD OCT 24 PY 2013 VL 357 BP 215 EP 222 DI 10.1016/j.chemgeo.2013.08.037 PG 8 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA 246WT UT WOS:000326572300019 ER PT J AU Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, C Rohringer, H Schofbeck, R Strauss, J Taurok, A Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, M Bansal, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Luyckx, S Mucibello, L Ochesanu, S Roland, B Rougny, R Staykova, Z Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Kalogeropoulos, A Keaveney, J Maes, M Olbrechts, A Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Clerbaux, B De Lentdecker, G Favart, L Gay, 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CA CMS Collaboration TI Measurement of the production cross section for Z gamma -> nu(nu)over-bar gamma in pp collisions at root s=7 TeV and limits on ZZ gamma and Z gamma gamma triple gauge boson couplings SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering ID SECTOR; TEVATRON; LEP AB A measurement of the Z gamma -> nu(nu) over bar gamma cross section in pp collisions at root s = 7 TeV is presented, using data corresponding to an integrated luminosity of 5.0 fb(-1) collected with the CMS detector. This measurement is based on the observation of events with an imbalance of transverse energy in excess of 130 GeV and a single photon in the absolute pseudorapidity range vertical bar eta vertical bar < 1.4 with transverse energy above 145 GeV. The Z gamma -> nu<(nu)over bar>gamma production cross section is measured to be 21.1 +/- 4.2(stat.)+/- 4.3(syst.)+/- 0.5(lum.)fb, which agrees with the standard model prediction of 21.9 +/- 1.1 fb. The results are combined with the CMS measurement of Z gamma production in the l(+)l(-)gamma final state (where l is an electron or a muon) to yield the most stringent limits to date on triple gauge boson couplings. vertical bar h(3)(Z)vertical bar < 2.7 x 10(-3), vertical bar h(4)(Z)vertical bar < 1.3 x 10(-5) for ZZ gamma and vertical bar h(3)(gamma)vertical bar < 2.9 x 10(-3), vertical bar h(4)(gamma)vertical bar < 1.5 x 10(-5) for Z gamma gamma couplings. C1 [Chatrchyan, S.; Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Bergauer, T.; Dragicevic, M.; Eroe, J.; Fabjan, C.; Friedl, M.; Fruehwirth, R.; Ghete, V. 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M.; Fahim, A.; Hesari, H.; Jafari, A.; Khakzad, M.; Najafabadi, M. Mohammadi; Mehdiabadi, S. Paktinat; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; Colaleo, A.; Creanza, D.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; Marangelli, B.; My, S.; Nuzzo, S.; Pacifico, N.; Pompili, A.; Pugliese, G.; Selvaggi, G.; Silvestris, L.; Singh, G.; Venditti, R.; Verwilligen, P.; Zito, G.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; De Palma, M.; Marangelli, B.; Nuzzo, S.; Pompili, A.; Selvaggi, G.; Singh, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Cufflani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Meneghelli, M.; Montanari, A.; Navarria, F. L.; Odorici, F.; Perrotta, A.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cufflani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Meneghelli, M.; Navarria, F. L.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Albergo, S.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Albergo, S.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gallo, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.] Univ Florence, Florence, Italy. [Fabbri, F.; Benussi, L.; Bianco, S.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Fabbricatore, P.; Musenich, R.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Tosi, S.] Univ Genoa, Genoa, Italy. [Benaglia, A.; De Guio, F.; Di Matteo, L.; Fiorendi, S.; Gennai, S.; Ghezzi, A.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. 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T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Vanini, S.; Ventura, S.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Bisello, D.; Branca, A.; Carlin, R.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Vanini, S.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.; Lazzizzera, I.] Univ Trento Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Nappi, A.; Romeo, F.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Biasini, M.; Fano, L.; Lariccia, P.; Mantovani, G.; Nappi, A.; Romeo, F.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; D'Agnolo, R. T.; Dell'Orso, R.; Fiori, F.; Foa, L.; Giassi, A.; Grippo, M. T.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; D'Agnolo, R. T.; Fiori, F.; Foa, L.; Ligabue, F.; Vernieri, C.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Diemoz, M.; Grassi, M.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Soffi, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; Del Re, D.; Grassi, M.; Longo, E.; Margaroli, F.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Soffi, L.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Demaria, N.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Ortona, G.; Pastrone, N.; Pelliccioni, M.; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Casasso, S.; Costa, M.; Migliore, E.; Monaco, V.; Ortona, G.; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Montanino, D.; Penzo, A.; Schizzi, A.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Chang, S.; Kim, T. Y.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, J. E.; Kong, D. J.; Oh, Y. D.; Park, H.; Son, D. C.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, J. Y.; Kim, Zero J.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, T. J.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. S.; Kwon, E.; Lee, B.; Lee, J.; Lee, S.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Grigelionis, I.; Juodagalvis, A.] Vilnius State Univ, Vilnius, Lithuania. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Lopez-Fernandez, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.; Reyes-Santos, M. A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Bell, A. J.; Butler, P. H.; Doesburg, R.; Reucroft, S.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Asghar, M. I.; Butt, J.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Wolszczak, W.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Almeida, N.; Bargassa, P.; David, A.; Faccioli, P.; Ferreira Parracho, P. C.; Gallinaro, M.; Rodrigues Antunes, J.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Karjavin, V.; Konoplyanikov, V.; Kozlov, G.; Laney, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Evstyukhin, S.; Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Erofeeva, M.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Belyaev, A.; Boos, E.; Bunichev, V.; Dubinin, M.; Dudko, L.; Ershov, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Markina, A.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Ekmedzic, M.; Krpic, D.; Milosevic, J.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Ekmedzic, M.; Krpic, D.; Milosevic, J.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Alcaraz Maestre, J.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Navarro De Martino, E.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.; Willmott, C.] CIEMAT, E-28040 Madrid, Spain. [Albajar, C.; de Troconiz, J. F.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.; Piedra Gomez, J.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Chuang, S. H.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Graziano, A.; Jorda, C.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Sanchez, F. J. Munoz; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Sharma, A.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Bendavid, J.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Coarasa Perez, J. A.; Colafranceschi, S.; d'Enterria, D.; Dabrowski, A.; De Roeck, A.; De Visscher, S.; Di Guida, S.; Dobson, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Funk, W.; Georgiou, G.; Giffels, M.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Giunta, M.; Glege, F.; Garrido, R. Gomez-Reino; Gowdy, S.; Guida, R.; Hammer, J.; Hansen, M.; Harris, P.; Hartl, C.; Hinzmann, A.; Innocente, V.; Janot, P.; Karavakis, E.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lee, Y. -J.; Lourenco, C.; Magini, N.; Malberti, M.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moser, R.; Mulders, M.; Musella, P.; Nesvold, E.; Orsini, L.; Cortezon, E. Palencia; Perez, E.; Perrozzi, L.; Petrilli, A.; Pfeiffer, A.; Pierini, M.; Pimia, M.; Piparo, D.; Plagge, M.; Polese, G.; Quertenmont, L.; Racz, A.; Reece, W.; Rolandi, G.; Rovelli, C.; Rovere, M.; Sakulin, H.; Santanastasio, F.; Schaefer, C.; Schwick, C.; Segoni, I.; Sekmen, S.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Stoye, M.; Tsirou, A.; Veres, G. I.; Vlimant, J. R.; Woehri, H. K.; Worm, S. D.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Gabathuler, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bortignon, P.; Buchmann, M. A.; Casal, B.; Chanon, N.; Deisher, A.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eller, P.; Freudenreich, K.; Grab, C.; Hits, D.; Lecomte, P.; Lustermann, W.; Marini, A. C.; del Arbol, P. Martinez Ruiz; Mohr, N.; Moortgat, F.; Naegeli, C.; Nef, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pape, L.; Pauss, F.; Peruzzi, M.; Ronga, F. J.; Rossini, M.; Sala, L.; Sanchez, A. K.; Starodumov, A.; Stieger, B.; Takahashi, M.; Tauscher, L.; Thea, A.; Theofilatos, K.; Treille, D.; Urscheler, C.; Wallny, R.; Weber, H. A.] Swiss Fed Inst Technol, Inst Particle Phys, Zurich, Switzerland. [Amsler, C.; Chiochia, V.; Favaro, C.; Rikova, M. Ivova; Kilminster, B.; Mejias, B. Millan; Otiougova, P.; Robmann, P.; Snoek, H.; Taroni, S.; Tupputi, S.; Verzetti, M.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Li, S. W.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Dietz, C.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Suwonjandee, N.] Chulalongkorn Univ, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Karapinar, G.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey. [Bahtiyar, H.; Barlas, E.; Cankocak, K.; Gunaydin, Y. O.; Vardarli, F. I.; Yucel, M.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Natl Sci Ctr, Kharkov Inst Phys & Technol, Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Kreczko, L.; Metson, S.; Newbold, D. M.; Nirunpong, K.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Basso, L.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Jackson, J.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Womersley, W. J.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Bainbridge, R.; Buchmuller, O.; Burton, D.; Ling, D. Col; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.; Whyntie, T.] Univ London Imperial Coll Sci Technol & Med, London, England. [Chadwick, M.; Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; St John, J.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Bhattacharya, S.; Alimena, J.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Houtz, R.; Ko, W.; Kopecky, A.; Lander, R.; Mall, O.; Miceli, T.; Nelson, R.; Pellett, D.; Ricci-Tam, F.; Rutherford, B.; Searle, M.; Smith, J.; Squires, M.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Weber, M.; Andreev, V.; Cline, D.; Cousins, R.; Erhan, S.; Everaerts, P.; Farrell, C.; Felcini, M.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Rakness, G.; Schlein, P.; Takasugi, E.; Traczyk, P.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Liu, H.; Babb, J.; Clare, R.; Dinardo, M. E.; Ellison, J.; Gary, J. W.; Hanson, G.; Long, O. R.; Luthra, A.; Nguyen, H.; Paramesvaran, S.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sharma, V.; Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; Evans, D.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Macneill, I.; Mangano, B.; Padhi, S.; Palmer, C.; Petrucciani, G.; Pieri, M.; Sani, M.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bellan, R.; Campagnari, C.; D'Alfonso, M.; Danielson, T.; Flowers, K.; Geffert, P.; George, C.; Golf, F.; Incandela, J.; Justus, C.; Kalavase, P.; Kovalskyi, D.; Krutelyov, V.; Lowette, S.; Villalba, R. Magana; Mccoll, N.; Pavlunin, V.; Ribnik, J.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Di Marco, E.; Duarte, J.; Kcira, D.; Ma, Y.; Mott, A.; Newman, H. B.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Veverka, J.; Wilkinson, R.; Xie, S.; Yang, Y.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Liu, Y. F.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Eggert, N.; Gibbons, L. K.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Gutsche, O.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Klima, B.; Kunori, S.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Ratnikova, N.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Wu, W.; Yang, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Chen, M.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Drozdetskiy, A.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Remington, R.; Rinkevicius, A.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Hewamanage, S.; Lebolo, L. M.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Gleyzer, S. V.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Callner, J.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Lacroix, F.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Strom, D.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Sen, N.; Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Griffiths, S.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Newsom, C. R.; Ogul, H.; Onel, Y.; Ozok, F.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Giurgiu, G.; Gritsan, A. V.; Hu, G.; Maksimovic, P.; Swartz, M.; Whitbeck, A.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Kenny, R. P., III; Murray, M.; Noonan, D.; Sanders, S.; Stringer, R.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Peterman, A.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Bauer, G.; Busza, W.; Butz, E.; Cali, I. A.; Chan, M.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Kim, Y.; Klute, M.; Lai, Y. S.; Levin, A.; Luckey, P. D.; Ma, T.; Nahn, S.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Sung, K.; Velicanu, D.; Wolf, R.; Wyslouch, B.; Yang, M.; Yilmaz, Y.; Yoon, A. S.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; De Benedetti, A.; Franzoni, G.; Gude, A.; Haupt, J.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Sasseville, M.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Cremaldi, L. M.; Kroeger, R.; Perera, L.; Rahmat, R.; Sanders, D. A.; Summers, D.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Eads, M.; Suarez, R. Gonzalez; Keller, J.; Kravchenko, I.; Lazo-Flores, J.; Malik, S.; Meier, F.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Dolen, J.; Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Kumar, A.; Rappoccio, S.; Wan, Z.] SUNY Buffalo, Buffalo, NY 14260 USA. 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Lopes; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Raval, A.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zenz, S. C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Brownson, E.; Lopez, A.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA. [Alagoz, E.; Benedetti, D.; Bolla, G.; Bortoletto, D.; De Mattia, M.; Everett, A.; Hu, Z.; Jones, M.; Jung, K.; Koybasi, O.; Kress, M.; Leonardo, N.; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Marono, M. Vidal; Wang, F.; Xu, L.; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Guragain, S.; Parashar, N.] Purdue Univ Calumet, Hammond, LA USA. [Li, W.; Adair, A.; Akgun, B.; Ecklund, K. M.; Geurts, F. J. M.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; Covarelli, R.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Miner, D. C.; Petrillo, G.; Vishnevskiy, D.; Zielinski, M.] Univ Rochester, Rochester, NY 14627 USA. [Malik, S.; Bhatti, A.; Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Lath, A.; Panwalkar, S.; Park, M.; Patel, R.; Rekovic, V.; Robles, J.; Rose, K.; Salur, S.; Schnetzer, S.; Seitz, C.; Somalwar, S.; Stone, R.; Thomas, S.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Cerizza, G.; Hollingsworth, M.; Spanier, S.; Yang, Z. C.; York, A.] Univ Tennessee, Knoxville, TN USA. 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RI Leonidov, Andrey/P-3197-2014; vilar, rocio/P-8480-2014; Dahms, Torsten/A-8453-2015; da Cruz e Silva, Cristovao/K-7229-2013; Grandi, Claudio/B-5654-2015; Chinellato, Jose Augusto/I-7972-2012; Bernardes, Cesar Augusto/D-2408-2015; Raidal, Martti/F-4436-2012; Lazzizzera, Ignazio/E-9678-2015; Sen, Sercan/C-6473-2014; D'Alessandro, Raffaello/F-5897-2015; Belyaev, Alexander/F-6637-2015; Stahl, Achim/E-8846-2011; Calderon, Alicia/K-3658-2014; de la Cruz, Begona/K-7552-2014; Scodellaro, Luca/K-9091-2014; Josa, Isabel/K-5184-2014; Calvo Alamillo, Enrique/L-1203-2014; VARDARLI, Fuat Ilkehan/B-6360-2013; Manganote, Edmilson/K-8251-2013; Paulini, Manfred/N-7794-2014; Vogel, Helmut/N-8882-2014; Ferguson, Thomas/O-3444-2014; Benussi, Luigi/O-9684-2014; Russ, James/P-3092-2014; Bartalini, Paolo/E-2512-2014; Wolszczak, Weronika/N-3113-2013; Petrushanko, Sergey/D-6880-2012; Ligabue, Franco/F-3432-2014; Wulz, Claudia-Elisabeth/H-5657-2011; Dudko, Lev/D-7127-2012; Lokhtin, Igor/D-7004-2012; Montanari, Alessandro/J-2420-2012; Cerrada, Marcos/J-6934-2014; Venturi, Andrea/J-1877-2012; Marlow, Daniel/C-9132-2014; de Jesus Damiao, Dilson/G-6218-2012; Janssen, Xavier/E-1915-2013; Novaes, Sergio/D-3532-2012; Trocsanyi, Zoltan/A-5598-2009; Konecki, Marcin/G-4164-2015; Hernandez Calama, Jose Maria/H-9127-2015; Bedoya, Cristina/K-8066-2014; My, Salvatore/I-5160-2015; Matorras, Francisco/I-4983-2015; Ragazzi, Stefano/D-2463-2009; Rovelli, Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Leonidov, Andrey/M-4440-2013; Andreev, Vladimir/M-8665-2015; TUVE', Cristina/P-3933-2015; KIM, Tae Jeong/P-7848-2015; Azarkin, Maxim/N-2578-2015; Flix, Josep/G-5414-2012; Della Ricca, Giuseppe/B-6826-2013; Tomei, Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Paganoni, Marco/A-4235-2016; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Tinoco Mendes, Andre David/D-4314-2011; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Mundim, Luiz/A-1291-2012; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Ruiz, Alberto/E-4473-2011; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017 OI Dahms, Torsten/0000-0003-4274-5476; Grandi, Claudio/0000-0001-5998-3070; Chinellato, Jose Augusto/0000-0002-3240-6270; Lazzizzera, Ignazio/0000-0001-5092-7531; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Belyaev, Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506; Scodellaro, Luca/0000-0002-4974-8330; Calvo Alamillo, Enrique/0000-0002-1100-2963; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Ferguson, Thomas/0000-0001-5822-3731; Benussi, Luigi/0000-0002-2363-8889; Russ, James/0000-0001-9856-9155; Ligabue, Franco/0000-0002-1549-7107; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Dudko, Lev/0000-0002-4462-3192; Montanari, Alessandro/0000-0003-2748-6373; Cerrada, Marcos/0000-0003-0112-1691; de Jesus Damiao, Dilson/0000-0002-3769-1680; Novaes, Sergio/0000-0003-0471-8549; Trocsanyi, Zoltan/0000-0002-2129-1279; Konecki, Marcin/0000-0001-9482-4841; Hernandez Calama, Jose Maria/0000-0001-6436-7547; Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680; Matorras, Francisco/0000-0003-4295-5668; Ragazzi, Stefano/0000-0001-8219-2074; Rovelli, Tiziano/0000-0002-9746-4842; TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; Flix, Josep/0000-0003-2688-8047; Della Ricca, Giuseppe/0000-0003-2831-6982; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Paganoni, Marco/0000-0003-2461-275X; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Mundim, Luiz/0000-0001-9964-7805; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; FU Austrian de la Recherche Scientifique; Fonds voor Wetenschappelijk Onderzoek; CNPq; CAPES; FAPERJ; FAPESP; Bulgarian Ministry of Education and Science; CERN; Chinese Academy of Sciences; Ministry of Science and Technology; National Natural Science Foundation of China; Colombian Funding Agency (COLCIENCIAS); Croatian Ministry of Science, Education and Sport; Research Promotion Foundation, Cyprus; Ministry of Education and Research [SF0690030s09]; European Regional Development Fund, Estonia; Academy of Finland; Finnish Ministry of Education and Culture; Helsinki Institute of Physics; Institut National de Physique Nucleaire et de Physique des Particules / CNRS; Commissariat a l'Energie Atomique et aux Energies Alternatives / CEA, France; Bundesministerium fur Bildung und Forschung; Deutsche Forschungsgemeinschaft; Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; General Secretariat for Research and Technology, Greece; National Scientific Research Foundation; National Office for Research and Technology, Hungary; Department of Atomic Energy; Department of Science and Technology, India; Institute for Studies in Theoretical Physics and Mathematics, Iran; Science Foundation, Ireland; Istituto Nazionale di Fisica Nucleare, Italy; Korean Ministry of Education, Science and Technology; World Class University program of NRF, Republic of Korea; Lithuanian Academy of Sciences; CINVESTAV; CONACYT; SEP; UASLP-FAI; Ministry of Business, Innovation and Employment, New Zealand; Pakistan Atomic Energy Commission; Ministry of Science and Higher Education; National Science Centre, Poland; Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; Ministry of Education and Science of the Russian Federation; Federal Agency of Atomic Energy of the Russian Federation; Russian Academy of Sciences; Russian Foundation for Basic Research; Ministry of Education, Science and Technological Development of Serbia; Secretaria de Estado de Investigacion, Desarrollo e Innovacion; Programa Consolider-Ingenio, Spain; ETH Board; ETH Zurich; PSI; SNF; UniZH; Canton Zurich; SER; National Science Council, Taipei; Thailand Center of Excellence in Physics; Institute for the Promotion of Teaching Science and Technology of Thailand; Special Task Force for Activating Research; National Science and Technology Development Agency of Thailand; Scientific and Technical Research Council of Turkey; Turkish Atomic Energy Authority; Science and Technology Facilities Council, U.K.; US Department of Energy; US National Science Foundation; Marie-Curie programme; European Research Council; EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of Czech Republic; Council of Science and Industrial Research, India; Compagnia di San Paolo (Torino); HOMING PLUS programme of Foundation for Polish Science; EU, Regional Development Fund; Thalis and Aristeia programmes; EU-ESF; Greek NSRF FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centres and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: the Austrian de la Recherche Scientifique, and Fonds voor Wetenschappelijk Onderzoek; the Brazilian Funding Agencies (CNPq, CAPES, FAPERJ, and FAPESP); the Bulgarian Ministry of Education and Science; CERN; the Chinese Academy of Sciences, Ministry of Science and Technology, and National Natural Science Foundation of China; the Colombian Funding Agency (COLCIENCIAS); the Croatian Ministry of Science, Education and Sport; the Research Promotion Foundation, Cyprus; the Ministry of Education and Research, Recurrent financing contract SF0690030s09 and European Regional Development Fund, Estonia; the Academy of Finland, Finnish Ministry of Education and Culture, and Helsinki Institute of Physics; the Institut National de Physique Nucleaire et de Physique des Particules / CNRS, and Commissariat a l'Energie Atomique et aux Energies Alternatives / CEA, France; the Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft, and Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; the General Secretariat for Research and Technology, Greece; the National Scientific Research Foundation, and National Office for Research and Technology, Hungary; the Department of Atomic Energy and the Department of Science and Technology, India; the Institute for Studies in Theoretical Physics and Mathematics, Iran; the Science Foundation, Ireland; the Istituto Nazionale di Fisica Nucleare, Italy; the Korean Ministry of Education, Science and Technology and the World Class University program of NRF, Republic of Korea; the Lithuanian Academy of Sciences; the Mexican Funding Agencies (CINVESTAV, CONACYT, SEP, and UASLP-FAI); the Ministry of Business, Innovation and Employment, New Zealand; the Pakistan Atomic Energy Commission; the Ministry of Science and Higher Education and the National Science Centre, Poland; the Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; the Ministry of Education and Science of the Russian Federation, the Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences, and the Russian Foundation for Basic Research; the Ministry of Education, Science and Technological Development of Serbia; the Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio 2010, Spain; the Swiss Funding Agencies (ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER); the National Science Council, Taipei; the Thailand Center of Excellence in Physics, the Institute for the Promotion of Teaching Science and Technology of Thailand, Special Task Force for Activating Research and the National Science and Technology Development Agency of Thailand; the Scientific and Technical Research Council of Turkey, and Turkish Atomic Energy Authority; the Science and Technology Facilities Council, U.K.; the US Department of Energy, and the US National Science Foundation.; Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of Czech Republic; the Council of Science and Industrial Research, India; the Compagnia di San Paolo (Torino); the HOMING PLUS programme of Foundation for Polish Science, cofinanced by EU, Regional Development Fund; and the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF. NR 35 TC 3 Z9 3 U1 3 U2 94 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD OCT 24 PY 2013 IS 10 AR 164 DI 10.1007/JHEP10(2013)164 PG 30 WC Physics, Particles & Fields SC Physics GA 241TJ UT WOS:000326190500001 ER PT J AU Chen, L Alarcon-Llado, E Hettick, M Sharp, ID Lin, YJ Javey, A Ager, JW AF Chen, Le Alarcon-Llado, Esther Hettick, Mark Sharp, Ian D. Lin, Yongjing Javey, Ali Ager, Joel W. TI Reactive Sputtering of Bismuth Vanadate Photoanodes for Solar Water Splitting SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID VISIBLE-LIGHT IRRADIATION; PHOTOCATALYTIC PROPERTIES; BIVO4; EFFICIENT; OXIDATION; COMPOSITE; PHOTOELECTRODES; TEMPERATURE; DEPOSITION; MECHANISM AB Bismuth vanadate (BiVO4) has attracted increasing attention as a photoanode for photoelectrochemical (PEC) water splitting. It has a band gap in the visible light range (2.4-2.5 eV) and a valence band position suitable for driving water oxidation under illumination. While a number of methods have been used to make BiVO4 photoanodes, scalable thin film deposition has remained relatively underexplored. Here, we report the synthesis of BiVO4 thin films by reactive sputtering. The use of separate Bi and V sputtering targets allows control of the Bi/V ratio in the film. Under optimized, slightly V-rich conditions, monoclinic phase BiVO4 with photoactivity for water oxidation is obtained. The highest photocurrents, ca. 1 mA cm(-2) at the reversible O-2/H2O potential with simulated AM 1.5G illumination, are obtained with bilayer WO3/BiVO4, where the WO3 serves as a hole-blocking layer. C1 [Chen, Le; Alarcon-Llado, Esther; Hettick, Mark; Sharp, Ian D.; Lin, Yongjing; Javey, Ali; Ager, Joel W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA. [Chen, Le; Alarcon-Llado, Esther; Hettick, Mark; Lin, Yongjing; Javey, Ali; Ager, Joel W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Sharp, Ian D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Alarcon-Llado, Esther] Ecole Polytech Fed Lausanne, Lausanne, Switzerland. [Hettick, Mark; Lin, Yongjing; Javey, Ali] Univ Calif Berkeley, Dept Elect Engn & Comp Sci, Berkeley, CA 94720 USA. RP Ager, JW (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, MS62R0203,1 Cyclotron Rd, Berkeley, CA 94720 USA. EM JWAger@lbl.gov RI Sharp, Ian/I-6163-2015; Javey, Ali/B-4818-2013; OI Sharp, Ian/0000-0001-5238-7487; Ager, Joel/0000-0001-9334-9751; Alarcon Llado, Esther/0000-0001-7317-9863 FU Office of Science of the U.S. Department of Energy [DE-SC0004993]; Marie Curie Actions Program FX This material is based upon work performed by the Joint Center for Artificial Photosynthesis, a DOE Energy Innovation Hub, supported through the Office of Science of the U.S. Department of Energy under Award Number DE-SC0004993. E.A.L. also acknowledges fellowship support from Marie Curie Actions Program. NR 36 TC 52 Z9 52 U1 6 U2 101 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD OCT 24 PY 2013 VL 117 IS 42 BP 21635 EP 21642 DI 10.1021/jp406019r PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 242RP UT WOS:000326260000002 ER PT J AU Choi, WI Wood, BC Schwegler, E Ogitsu, T AF Choi, Woon Ih Wood, Brandon C. Schwegler, Eric Ogitsu, Tadashi TI Site-Dependent Free Energy Barrier for Proton Reduction on MoS2 Edges SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID HYDROGEN EVOLUTION; SOLAR-ENERGY; ELECTROCATALYSIS; NANOCATALYSTS; NANOPARTICLES; NANOCLUSTERS; CATALYST; CELLS AB We calculated the adiabatic free energy surface of the proton reduction reaction on catalytically active MoS2 edge atoms by combining density functional theory with the Anderson-Newns model, which accounts for solvent fluctuation and charge transfer in the context of Marcus theory. This framework combines three different contributions to the associated reaction energetics and kinetics, namely, the relevant electronic orbitals of the substrate, the possibility of surface relaxation upon adsorption, and the impact of solvation. Under the assumption of fixed edge geometry throughout the reaction, we calculate the free energy barriers on edge S and Mo sites to be 0.65 and 0 eV, respectively. However, if we consider surface relaxation, the barrier on the edge S site is reduced by more than half to 0.31 eV. On edge Mo sites, the d(z)(2) orbital is responsible not only for the strength of binding but also for the barrierless reaction. On edge S sites, the bound hydrogen atom always retains some finite positive charge, which indicates that it remains partially solvated even after surface binding. In this case, it is crucial to account for the solvation energy in addition to the gas-phase adsorption energy when assessing hydrogen catalysis. C1 [Choi, Woon Ih; Wood, Brandon C.; Schwegler, Eric; Ogitsu, Tadashi] Lawrence Livermore Natl Lab, Quantum Simulat Grp, Livermore, CA 94550 USA. RP Ogitsu, T (reprint author), Lawrence Livermore Natl Lab, Quantum Simulat Grp, Livermore, CA 94550 USA. EM ogitsu1@llnl.gov RI Schwegler, Eric/A-2436-2016; OI Schwegler, Eric/0000-0003-3635-7418; Choi, Woon Ih/0000-0002-7183-3400 FU U.S. Department of Energy Fuel Cell Technologies Program; Laboratory Directed Research and Development (LDRD) Program of Lawrence Livermore National Laboratory (LLNL); U.S. Department of Energy by LLNL [DE-AC52-07NA27344] FX The authors acknowledge helpful discussions with E. Santos (U. of Ulm, Germany). We also gratefully acknowledge funding support from the U.S. Department of Energy Fuel Cell Technologies Program and Laboratory Directed Research and Development (LDRD) Program of Lawrence Livermore National Laboratory (LLNL). Computing support came from the Lawrence Livermore National Laboratory (LLNL) Institutional Computing Grand Challenge program. This work was performed under the auspices of the U.S. Department of Energy by LLNL under Contract DE-AC52-07NA27344. NR 31 TC 11 Z9 13 U1 1 U2 43 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 EI 1932-7455 J9 J PHYS CHEM C JI J. Phys. Chem. C PD OCT 24 PY 2013 VL 117 IS 42 BP 21772 EP 21777 DI 10.1021/jp405354u PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 242RP UT WOS:000326260000017 ER PT J AU Alayoglu, S Beaumont, SK Melaet, G Lindeman, AE Musselwhite, N Brooks, CJ Marcus, MA Guo, JG Liu, Z Kruse, N Somorjai, GA AF Alayoglu, Selim Beaumont, Simon K. Melaet, Gerome Lindeman, Avery E. Musselwhite, Nathan Brooks, Christopher J. Marcus, Matthew A. Guo, Jingua Liu, Zhi Kruse, Norbert Somorjai, Gabor A. TI Surface Composition Changes of Redox Stabilized Bimetallic CoCu Nanoparticles Supported on Silica under H-2 and O-2 Atmospheres and During Reaction between CO2 and H-2: In Situ X-ray Spectroscopic Characterization SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID FISCHER-TROPSCH SYNTHESIS; METHANOL SYNTHESIS; PHOTOELECTRON-SPECTROSCOPY; SYNTHESIS CATALYSTS; COBALT CATALYSTS; HYDROGENATION; SELECTIVITY; KINETICS; SCIENCE; DESIGN AB In this paper, we report the colloidal synthesis and detailed characterization of 11 nm bimetallic CoCu nanoparticle catalysts. Presently Co and Cu is an attractive combination because of their respective properties for industrially important Fischer-Tropsch and methanol synthesis reactions of CO (and CO2) with H-2. We report the preparation of catalysts by deposition of bimetallic metal nanoparticles, both within mesoporous silica (MCF-17) and on the native oxide surface of a silicon wafer. Subsequent phase separation into phase-segregated (i.e., dimer) particles is found to occur upon redox treatment. These nanoparticle catalysts have then been investigated using an array of techniques including synchrotron-based ambient pressure X-ray photoelectron spectroscopy (APXPS) and in situ near edge and extended X-ray absorption fine structure (NEXAFS/EXAFS) spectroscopies. CO2 hydrogenation is used as a probe reaction. All three techniques combine to show that an oxygen atmosphere segregates copper to the surface. In doing so the oxygen produces oxides of both Co and Cu metals. Significant hydrogen pressure and temperature are required to fully rereduce both metals to a metallic state as demonstrated by NEXAFS spectroscopy. Under the conditions of the CO2/H-2 reaction monitored in situ using NEXAFS spectroscopy, both metals exist in a fully reduced state at 2.7 bar, 1:3 CO2:H-2, and 260 degrees C. C1 [Alayoglu, Selim; Beaumont, Simon K.; Melaet, Gerome; Lindeman, Avery E.; Musselwhite, Nathan; Somorjai, Gabor A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94704 USA. [Alayoglu, Selim; Beaumont, Simon K.; Melaet, Gerome; Lindeman, Avery E.; Musselwhite, Nathan; Somorjai, Gabor A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Brooks, Christopher J.] Honda Res Inst, Columbus, OH 43212 USA. [Marcus, Matthew A.; Guo, Jingua; Liu, Zhi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Kruse, Norbert] Univ Libre Bruxelles, B-1050 Brussels, Belgium. RP Somorjai, GA (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94704 USA. EM somorjai@berkeley.edu RI Liu, Zhi/B-3642-2009; Melaet, Gerome/N-4879-2015; Foundry, Molecular/G-9968-2014; Beaumont, Simon/F-5272-2012 OI Liu, Zhi/0000-0002-8973-6561; Melaet, Gerome/0000-0003-1414-1683; Beaumont, Simon/0000-0002-1973-9783 FU Office of Energy Research, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231]; Honda Research Institute, USA FX The user projects in the Advanced Light Source and Molecular Foundry at the Lawrence Berkeley National Laboratory were supported by the Director, Office of Energy Research, Office of Basic Energy Sciences of the U.S. Department of Energy under Contract DE-AC02-05CH11231. We acknowledge Honda Research Institute, USA for the financial support. NR 36 TC 14 Z9 14 U1 3 U2 59 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD OCT 24 PY 2013 VL 117 IS 42 BP 21803 EP 21809 DI 10.1021/jp405745n PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 242RP UT WOS:000326260000021 ER PT J AU Wong, CY Penwell, SB Cotts, BL Noriega, R Wu, H Ginsberg, NS AF Wong, Cathy Y. Penwell, Samuel B. Cotts, Benjamin L. Noriega, Rodrigo Wu, Hao Ginsberg, Naomi S. TI Revealing Exciton Dynamics in a Small-Molecule Organic Semiconducting Film with Subdomain Transient Absorption Microscopy SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID PUMP-PROBE SPECTROSCOPY; CHARGE-TRANSFER STATE; SOLAR-CELLS; FUNCTIONALIZED PENTACENE; SINGLET FISSION; ULTRAFAST DYNAMICS; QUANTUM EFFICIENCY; PHOTOVOLTAIC CELLS; POLYMER BLENDS; FREE-CARRIER AB The ultrafast spectroscopy of single domains of polycrystalline films of TIPS-pentacene, a small-molecule organic semiconductor of interest in electronic and photovoltaic applications, is investigated using transient absorption microscopy. Individual domains are distinguished by their different polarization-dependent linear and nonlinear optical responses. As compared to bulk measurements, we show that the nonlinear response within a given domain can be tied more concretely to specific physical processes that transfer exciton populations between specified electronic states. By use of this approach and a simple kinetic model, the signatures of singlet fission as well as vibrational relaxation of the initially excited singlet state are identified. As such, observing exciton dynamics within and comparing exciton dynamics between different TIPS-pentacene domains reveal the relationship between photophysics and film morphology needed to improve device performance. C1 [Wong, Cathy Y.; Penwell, Samuel B.; Cotts, Benjamin L.; Noriega, Rodrigo; Wu, Hao; Ginsberg, Naomi S.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Ginsberg, Naomi S.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Ginsberg, Naomi S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci & Mat Sci Div, Berkeley, CA 94720 USA. [Ginsberg, Naomi S.] Kavli Energy NanoSci Inst, Berkeley, CA 94720 USA. RP Ginsberg, NS (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM nsginsberg@berkeley.edu FU Defense Advanced Research Projects Agency Young Faculty Award [N66001-12-1-4228]; Natural Sciences and Engineering Research Council, Canada; Department of Energy Office of Science Graduate Research Fellowship [DE-AC05-060R23100]; National Science Foundation Graduate Research Fellowship [DGE 1106400]; Philomathia Foundation; David and Lucile Packard Foundation Fellowship for Science and Engineering FX This work has been supported by the Defense Advanced Research Projects Agency Young Faculty Award number N66001-12-1-4228. C.Y.W. thanks the Natural Sciences and Engineering Research Council, Canada, for a Postdoctoral Fellowship. S.B.P. acknowledges a Department of Energy Office of Science Graduate Research Fellowship, made possible in part by the American Recovery and Reinvestment Act of 2009, administered by ORISE-ORAU under contract no. DE-AC05-060R23100; B.L.C. acknowledges a National Science Foundation Graduate Research Fellowship (DGE 1106400); RN. acknowledges the Philomathia Foundation for support; and N.S.G. acknowledges a David and Lucile Packard Foundation Fellowship for Science and Engineering. We also thank V. Ho and R. Segalman for advice in sample preparation. NR 91 TC 24 Z9 24 U1 10 U2 97 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 EI 1932-7455 J9 J PHYS CHEM C JI J. Phys. Chem. C PD OCT 24 PY 2013 VL 117 IS 42 BP 22111 EP 22122 DI 10.1021/jp407645k PG 12 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 242RP UT WOS:000326260000059 ER PT J AU Petkov, V Shastri, S Shan, SY Joseph, P Luo, J Zhong, CJ Nakamura, T Herbani, Y Sato, S AF Petkov, Valeri Shastri, Sarvjit Shan, Shiyao Joseph, Pharrah Luo, Jin Zhong, Chuan-Jian Nakamura, Takahiro Herbani, Yuliati Sato, Shunichi TI Resolving Atomic Ordering Differences in Group 11 Nanosized Metals and Binary Alloy Catalysts by Resonant High-Energy X-ray Diffraction and Computer Simulations SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID INTERMETALLIC COMPOUNDS; SOLID-SOLUTIONS; SHORT-RANGE; NANOPARTICLES; PARTICLES; CRYSTALS; SIZE; NANOCLUSTERS; OXIDATION; SURFACES AB Resonant high-energy X-ray diffraction coupled to atomic pair distribution function analysis and computer simulations is used to study the atomic-scale structure of group 11 nanosized metals and binary alloy catalysts. We find that nanosized Cu is quite disordered structurally whereas nanosized Ag and especially Au exhibit a very good degree of crystallinity. We resolve CuCu and AgAg atomic correlations from Au-involving ones in AuCu and AuAg nanoalloys and show that depending on the synthetic route group 11 binary alloys may adopt structural states that obey or markedly violate Vegards law. In the latter case, Cu and Ag atoms undergo substantial size expansion and contraction by as much as 0.3 and 0.03 angstrom, respectively, while heavier Au atoms remain practically intact. The size change of Cu and Ag atoms does not follow Paulings rule of electronegativity predicting charge flow toward the more electronegative Au but occurs in a way such that Cu/Au and Ag/Au atomic size ratios in the nanoalloys become closer to one. Atomic size adjusting and the concurrent charge redistribution result in a synergistic effect of oxygen inactive Au and oxygen very active Cu and Ag leading to nanoalloys with very good activity for low-temperature oxidation of CO. C1 [Petkov, Valeri] Cent Michigan Univ, Dept Phys, Mt Pleasant, MI 48859 USA. [Shastri, Sarvjit] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Shan, Shiyao; Joseph, Pharrah; Luo, Jin; Zhong, Chuan-Jian] SUNY Binghamton, Dept Chem, Binghamton, NY 13902 USA. [Nakamura, Takahiro; Sato, Shunichi] Tohoku Univ, Inst Multidisciplinary Res Adv Mat, Aoba Ku, Sendai, Miyagi 9808577, Japan. [Herbani, Yuliati] Indonesian Inst Sci, Res Ctr Phys, Serpong 15314, Tangerang Bante, Indonesia. RP Petkov, V (reprint author), Cent Michigan Univ, Dept Phys, Mt Pleasant, MI 48859 USA. EM petko1vg@cmich.edu RI Zhong, Chuan-Jian/D-3394-2013 FU DOE-BES [DE-SC0006877]; DOE [DEAC02-06CH11357] FX Work on this paper was supported by DOE-BES Grant DE-SC0006877. Work at the Advanced Photon Source was supported by DOE under Contract DEAC02-06CH11357. NR 44 TC 12 Z9 12 U1 4 U2 26 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD OCT 24 PY 2013 VL 117 IS 42 BP 22131 EP 22141 DI 10.1021/jp408017v PG 11 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 242RP UT WOS:000326260000061 ER PT J AU Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Eroe, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, C Rohringer, H Schofbeck, R Strauss, J Taurok, A Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, M Bansal, S Cornelis, T DeWolf, EA Janssen, X Knutsson, A Luyckx, S Mucibello, L Ochesanu, S Roland, B Rougny, R Staykova, Z Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Kalogeropoulos, A Keaveney, J Maes, M Olbrechts, A Tavernier, 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Sarangi, T. Savin, A. Smith, W. H. Swanson, J. CA CMS Collaboration TI Measurement of the W-boson helicity in top-quark decays from t(t)over-bar production in lepton plus jets events in pp collisions at root s=7 TeV SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering; Top physics ID ANOMALOUS WTB COUPLINGS; PARTON DISTRIBUTIONS; LHC; FRACTIONS AB The W-boson helicity fractions in top-quark decays are measured with t (t) over bar events in the lepton+jets final state, using proton-proton collisions at a centre-of-mass energy of 7 TeV, collected in 2011 with the CMS detector at the LHC. The data sample corresponds to an integrated luminosity of 5.0 fb(-1). The measured fractions of longitudinal, left-, and right-handed helicity are F-0 = 0.682 +/- 0.030 (stat.) +/- 0.033 (syst.), F-L = 0.310 +/- 0.022 (stat.) +/- 0.022 (syst.), and F-R = 0.008 +/- 0.012 (stat.) +/- 0.014 (syst.), consistent with the standard model predictions. 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[Horvath, D.; Beni, N.; Czellar, S.; Molnar, J.; Palinkas, J.; Szillasi, Z.; Abdulsalam, A.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Karancsi, J.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, H-4012 Debrecen, Hungary. [Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Beri, S. B.; Bhatnagar, V.; Dhingra, N.; Gupta, R.; Kaur, M.; Mehta, M. Z.; Mittal, M.; Nishu, N.; Sharma, A.; Singh, J. B.] Panjab Univ, Chandigarh 160014, India. [Kumar, Ashok; Kumar, Arun; Ahuja, S.; Bhardwaj, A.; Choudhary, B. C.; Malhotra, S.; Naimuddin, M.; Ranjan, K.; Saxena, P.; Sharma, V.; Shivpuri, R. K.] Univ Delhi, Delhi 110007, India. [Banerjee, S.; Bhattacharya, S.; Chatterjee, K.; Dutta, S.; Gomber, B.; Jain, Sa.; Jain, Sh.; Khurana, R.; Modak, A.; Mukherjee, S.; Roy, D.; Sarkar, S.; Sharan, M.; Singh, A. P.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Dutta, D.; Kailas, S.; Kumar, V.; Mohanty, A. K.; Pant, L. 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S.; Colaleo, A.; Creanza, D.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; Marangelli, B.; My, S.; Nuzzo, S.; Pacifico, N.; Pompili, A.; Pugliese, G.; Selvaggi, G.; Silvestris, L.; Singh, G.; Venditti, R.; Verwilligen, P.; Zito, G.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; De Palma, M.; Marangelli, B.; Nuzzo, S.; Pompili, A.; Selvaggi, G.; Singh, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Meneghelli, M.; Montanari, A.; Navarria, F. 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[Ciulli, V.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gonzi, S.; Lenzi, P.; Tropiano, A.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Fabbri, F.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Fabbricatore, P.; Ferretti, R.; Ferro, F.; Lo Vetere, M.; Musenich, R.; Robutti, E.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Ferretti, R.; Lo Vetere, M.; Tosi, S.] Univ Genoa, Genoa, Italy. [Benaglia, A.; Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] Ist Nazl Fis Nucl, Sez Milano Bicocca, I-20133 Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Manzoni, R. A.; Martelli, A.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; De Cosa, A.; Fabozzi, F.; Iorio, A. O. M.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [De Cosa, A.; Iorio, A. O. M.] Univ Naples Federico II, Naples, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata Potenza, Naples, Italy. [Meola, S.] Univ G Marconi Roma, Naples, Italy. [Azzi, P.; Bacchetta, N.; Bellato, M.; Branca, A.; Carlin, R.; Checchia, P.; Dorigo, T.; Dosselli, U.; Fanzago, F.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Lazzizzera, I.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pegoraro, M.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Triossi, A.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Bisello, D.; Branca, A.; Carlin, R.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Margoni, M.; Meneguzzo, A. 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T.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Moon, C. S.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; D'Agnolo, R. T.; Fiori, F.; Foa, L.; Ligabue, F.; Vernieri, C.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Diemoz, M.; Grassi, M.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Rovelli, C.; Soffi, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; Del Re, D.; Grassi, M.; Longo, E.; Margaroli, F.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Soffi, L.] Univ Rome, Rome, Italy. [Costa, S.; Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Casasso, S.; Degano, A.; Demaria, N.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Pastrone, N.; Pelliccioni, M.; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Arneodo, M.; Bellan, R.; Casasso, S.; Costa, M.; Degano, A.; Migliore, E.; Monaco, V.; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Montanino, D.; Penzo, A.; Schizzi, A.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Chang, S.; Kim, T. Y.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, J. E.; Kong, D. J.; Lee, S.; Oh, Y. D.; Park, H.; Son, D. C.; Kamon, T.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, J. Y.; Kim, Zero J.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, T. J.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. S.; Kwon, E.; Lee, B.; Lee, J.; Lee, S.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Grigelionis, I.; Juodagalvis, A.] Vilnius State Univ, Vilnius, Lithuania. [Castilla-Valdez, H.; De la Cruz-Burelo, E.; Heredia-de La Cruz, I.; Lopez-Fernandez, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.; Reyes-Santos, M. A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Doesburg, R.; Reucroft, S.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Asghar, M. I.; Butt, J.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. 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[Popov, A.; Zhukov, V.; Katkov, I.; Belyaev, A.; Boos, E.; Bunichev, V.; Dubinin, M.; Dudko, L.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Markina, A.; Obraztsov, S.; Perfilov, M.; Savrin, V.; Tsirova, N.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. 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Palencia; Perez, E.; Perrozzi, L.; Petrilli, A.; Pfeiffer, A.; Pierini, M.; Pimia, M.; Piparo, D.; Plagge, M.; Quertenmont, L.; Racz, A.; Reece, W.; Rolandi, G.; Rovere, M.; Sakulin, H.; Santanastasio, F.; Schaefer, C.; Schwick, C.; Segoni, I.; Sekmen, S.; Sharma, A.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Stoye, M.; Tsirou, A.; Veres, G. I.; Vlimant, J. R.; Woehri, H. K.; Worm, S. D.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Gabathuler, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Bortignon, P.; Buchmann, M. A.; Casal, B.; Chanon, N.; Deisher, A.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eller, P.; Freudenreich, K.; Grab, C.; Hits, D.; Lecomte, P.; Lustermann, W.; Mangano, B.; Marini, A. C.; del Arbol, P. Martinez Ruiz; Meister, D.; Mohr, N.; Moortgat, F.; Naegeli, C.; Nef, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pape, L.; Pauss, F.; Peruzzi, M.; Ronga, F. J.; Rossini, M.; Sala, L.; Sanchez, A. K.; Starodumov, A.; Stieger, B.; Takahashi, M.; Tauscher, L.; Thea, A.; Theofilatos, K.; Treille, D.; Urscheler, C.; Wallny, R.; Weber, H. A.] Swiss Fed Inst Technol, Inst Particle Phys, Zurich, Switzerland. [Amsler, C.; Chiochia, V.; Favaro, C.; Rikova, M. Ivova; Kilminster, B.; Mejias, B. Millan; Robmann, P.; Snoek, H.; Taroni, S.; Verzetti, M.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Li, S. W.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Dietz, C.; Grundler, U.; Hou, W-S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Lu, R-S.; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Suwonjandee, N.] Chulalongkorn Univ, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Karapinar, G.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey. [Bahtiyar, H.; Barlas, E.; Cankocak, K.; Gunaydin, Y. O.; Vardarli, F. I.; Yucel, M.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Kreczko, L.; Lucas, C.; Meng, Z.; Metson, S.; Newbold, D. M.; Nirunpong, K.; Paramesvaran, S.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Worm, S. D.; Newbold, D. M.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Radburn-Smith, C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Womersley, W. J.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A-M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.] Univ London Imperial Coll Sci Technol & Med, London, England. [Chadwick, M.; Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; St John, J.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Bhattacharya, S.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De la Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Houtz, R.; Ko, W.; Kopecky, A.; Lander, R.; Miceli, T.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Rutherford, B.; Searle, M.; Smith, J.; Squires, M.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Andreev, V.; Cline, D.; Cousins, R.; Erhan, S.; Everaerts, P.; Farrell, C.; Felcini, M.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Rakness, G.; Schlein, P.; Takasugi, E.; Traczyk, P.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Babb, J.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Jandir, P.; Liu, H.; Long, O. R.; Luthra, A.; Malberti, M.; Nguyen, H.; Shrinivas, A.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; Evans, D.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Macneill, I.; Padhi, S.; Palmer, C.; Petrucciani, G.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Campagnari, C.; Danielson, T.; Flowers, K.; Geffert, P.; George, C.; Golf, F.; Incandela, J.; Justus, C.; Kovalskyi, D.; Krutelyov, V.; Lowette, S.; Villalba, R. Magana; Mccoll, N.; Pavlunin, V.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dias, F. A.; Dubinin, M.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Di Marco, E.; Duarte, J.; Kcira, D.; Ma, Y.; Mott, A.; Newman, H. B.; Pena, C.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Veverka, J.; Wilkinson, R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Liu, Y. F.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Eggert, N.; Gibbons, L. K.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Gutsche, O.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Kaadze, K.; Klima, B.; Kunori, S.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Ratnikova, N.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Wu, W.; Yang, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Chen, M.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Drozdetskiy, A.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Remington, R.; Rinkevicius, A.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Gleyzer, S. V.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, Vic, Australia. [Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Callner, J.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Lacroix, F.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Strom, D.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Griffiths, S.; Merlo, P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Newsom, C. R.; Ogul, H.; Onel, Y.; Ozok, F.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Giurgiu, G.; Gritsan, A. V.; Hu, G.; Maksimovic, P.; Martin, C.; Swartz, M.; Whitbeck, A.] Johns Hopkins Univ, Baltimore, MD USA. [Sibille, J.; Baringer, P.; Bean, A.; Benelli, G.; Kenny, R. P., III; Murray, M.; Noonan, D.; Sanders, S.; Stringer, R.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Peterman, A.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Bauer, G.; Busza, W.; Cali, I. A.; Chan, M.; Di Matteo, L.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Kim, Y.; Klute, M.; Lai, Y. S.; Levin, A.; Luckey, P. D.; Ma, T.; Nahn, S.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Velicanu, D.; Wolf, R.; Wyslouch, B.; Yang, M.; Yilmaz, Y.; Yoon, A. S.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; De Benedetti, A.; Franzoni, G.; Gude, A.; Haupt, J.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Sasseville, M.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Cremaldi, L. M.; Kroeger, R.; Oliveros, S.; Perera, L.; Rahmat, R.; Sanders, D. A.; Summers, D.] Univ Mississippi, University, MS 38677 USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Eads, M.; Suarez, R. Gonzalez; Keller, J.; Kravchenko, I.; Lazo-Flores, J.; Malik, S.; Meier, F.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Dolen, J.; Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Kumar, A.; Rappoccio, S.; Wan, Z.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Massironi, A.; Nash, D.; Orimoto, T.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Anastassov, A.; Hahn, K. A.; Kubik, A.; Lusito, L.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Berry, D.; Brinkerhoff, A.; Chan, K. M.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kolb, J.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Morse, D. M.; Pearson, T.; Planer, M.; Ruchti, R.; Slaunwhite, J.; Valls, N.; Wayne, M.; Wolf, M.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Bylsma, B.; Durkin, L. S.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Puigh, D.; Rodenburg, M.; Smith, G.; Vuosalo, C.; Winer, B. L.; Wolfe, H.] Ohio State Univ, Columbus, OH 43210 USA. [Berry, E.; Elmer, P.; Halyo, V.; Hebda, P.; Hegeman, J.; Hunt, A.; Jindal, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Raval, A.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zenz, S. C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Brownson, E.; Lopez, A.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA. [Savoy-Navarro, A.; Alagoz, E.; Benedetti, D.; Bolla, G.; Bortoletto, D.; De Mattia, M.; Everett, A.; Hu, Z.; Jones, M.; Jung, K.; Koybasi, O.; Kress, M.; Leonardo, N.; Pegna, D. Lopes; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Marono, M. Vidal; Wang, F.; Xie, W.; Xu, L.; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Ecklund, K. M.; Geurts, F. J. M.; Li, W.; Michlin, B.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; Covarelli, R.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Miner, D. C.; Petrillo, G.; Vishnevskiy, D.; Zielinski, M.] Univ Rochester, Rochester, NY 14627 USA. [Bhatti, A.; Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Malik, S.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Lath, A.; Panwalkar, S.; Park, M.; Patel, R.; Rekovic, V.; Robles, J.; Salur, S.; Schnetzer, S.; Seitz, C.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Cerizza, G.; Hollingsworth, M.; Rose, K.; Spanier, S.; Yang, Z. C.; York, A.] Univ Tennessee, Knoxville, TN USA. [Bouhali, O.; Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Khotilovich, V.; Montalvo, R.; Osipenkov, I.; Pakhotin, Y.; Perloff, A.; Roe, J.; Safonov, A.; Sakuma, T.; Suarez, I.; Tatarinov, A.; Toback, D.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Kovitanggoon, K.; Lee, S. W.; Libeiro, T.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Johns, W.; Maguire, C.; Mao, Y.; Melo, A.; Sharma, M.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN 37235 USA. [Arenton, M. W.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Lin, C.; Neu, C.; Wood, J.] Univ Virginia, Charlottesville, VA USA. [Gollapinni, S.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sakharov, A.] Wayne State Univ, Detroit, MI USA. [Belknap, D. A.; Borrello, L.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Duric, S.; Friis, E.; Grothe, M.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Klukas, J.; Lanaro, A.; Loveless, R.; Mohapatra, A.; Mozer, M. U.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ross, I.; Sarangi, T.; Savin, A.; Smith, W. H.; Swanson, J.] Univ Wisconsin, Madison, WI 53706 USA. [Fabjan, C.; Jeitler, M.; Krammer, M.; Wulz, C-E.] Vienna Univ Technol, A-1040 Vienna, Austria. [Chinellato, J.; Tonelli Manganote, E. J.] Univ Estadual Campinas, Campinas, SP, Brazil. [Assran, Y.] Suez Canal Univ, Suez, Egypt. Zewail City Sci & Technol, Zewail, Egypt. Cairo Univ, Cairo, Egypt. [Awad, A. M. Kuotb; Mahmoud, M. A.] Fayoum Univ, Al Fayyum, Egypt. [Radi, A.] British Univ Egypt, Cairo, Egypt. [Agram, J-L.; Conte, E.; Drouhin, F.; Fontaine, J-C.] Univ Haute Alsace, Mulhouse, France. [Bergholz, M.; Lohmann, W.; Schmidt, R.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Veres, G. 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[Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Kaya, M.; Kaya, O.] Kafkas Univ, Kars, Turkey. [Ozkorucuklu, S.] Suleyman Demirel Univ, TR-32200 Isparta, Turkey. [Sonmez, N.] Ege Univ, Izmir, Turkey. [Bahtiyar, H.; Albayrak, E. A.; Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Gunaydin, Y. O.] Kahramanmaras Sutcu Imam Univ, Kahramanmaras, Turkey. [Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Wasserbaech, S.] Utah Valley Univ, Orem, UT USA. [Bilki, B.] Argonne Natl Lab, Argonne, IL 60439 USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Yetkin, T.] Yildiz Tekn Univ, Istanbul, Turkey. [Bouhali, O.] Texas A& M Univ Qatar, Doha, Qatar. RP Chatrchyan, S (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Tomei, Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Paganoni, Marco/A-4235-2016; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Sznajder, Andre/L-1621-2016; Vilela Pereira, Antonio/L-4142-2016; Mundim, Luiz/A-1291-2012; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Ruiz, Alberto/E-4473-2011; Lo Vetere, Maurizio/J-5049-2012; Ragazzi, Stefano/D-2463-2009; Rovelli, Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Leonidov, Andrey/M-4440-2013; Andreev, Vladimir/M-8665-2015; TUVE', Cristina/P-3933-2015; KIM, Tae Jeong/P-7848-2015; Azarkin, Maxim/N-2578-2015; Flix, Josep/G-5414-2012; Della Ricca, Giuseppe/B-6826-2013; Lazzizzera, Ignazio/E-9678-2015; Sen, Sercan/C-6473-2014; D'Alessandro, Raffaello/F-5897-2015; Belyaev, Alexander/F-6637-2015; Stahl, Achim/E-8846-2011; Trocsanyi, Zoltan/A-5598-2009; Konecki, Marcin/G-4164-2015; Hernandez Calama, Jose Maria/H-9127-2015; ciocci, maria agnese /I-2153-2015; Bedoya, Cristina/K-8066-2014; My, Salvatore/I-5160-2015; Matorras, Francisco/I-4983-2015; Manganote, Edmilson/K-8251-2013; Paulini, Manfred/N-7794-2014; Vogel, Helmut/N-8882-2014; Ferguson, Thomas/O-3444-2014; Benussi, Luigi/O-9684-2014; Russ, James/P-3092-2014; Leonidov, Andrey/P-3197-2014; vilar, rocio/P-8480-2014; Dahms, Torsten/A-8453-2015; Grandi, Claudio/B-5654-2015; Chinellato, Jose Augusto/I-7972-2012; Bernardes, Cesar Augusto/D-2408-2015; Raidal, Martti/F-4436-2012; Lokhtin, Igor/D-7004-2012; Montanari, Alessandro/J-2420-2012; Moon, Chang-Seong/J-3619-2014; Gribushin, Andrei/J-4225-2012; Cerrada, Marcos/J-6934-2014; Venturi, Andrea/J-1877-2012; Calderon, Alicia/K-3658-2014; de la Cruz, Begona/K-7552-2014; Scodellaro, Luca/K-9091-2014; Josa, Isabel/K-5184-2014; Calvo Alamillo, Enrique/L-1203-2014; VARDARLI, Fuat Ilkehan/B-6360-2013; Wolszczak, Weronika/N-3113-2013; Tinoco Mendes, Andre David/D-4314-2011; Novaes, Sergio/D-3532-2012; Bartalini, Paolo/E-2512-2014; Santoro, Alberto/E-7932-2014; Ligabue, Franco/F-3432-2014; Wulz, Claudia-Elisabeth/H-5657-2011; Dudko, Lev/D-7127-2012; Codispoti, Giuseppe/F-6574-2014; da Cruz e Silva, Cristovao/K-7229-2013; Marlow, Daniel/C-9132-2014; de Jesus Damiao, Dilson/G-6218-2012; Janssen, Xavier/E-1915-2013; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017 OI Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Paganoni, Marco/0000-0003-2461-275X; Gulmez, Erhan/0000-0002-6353-518X; Sznajder, Andre/0000-0001-6998-1108; Vilela Pereira, Antonio/0000-0003-3177-4626; Mundim, Luiz/0000-0001-9964-7805; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Lo Vetere, Maurizio/0000-0002-6520-4480; Ragazzi, Stefano/0000-0001-8219-2074; Rovelli, Tiziano/0000-0002-9746-4842; TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; Flix, Josep/0000-0003-2688-8047; Della Ricca, Giuseppe/0000-0003-2831-6982; Lazzizzera, Ignazio/0000-0001-5092-7531; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Belyaev, Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279; Konecki, Marcin/0000-0001-9482-4841; Hernandez Calama, Jose Maria/0000-0001-6436-7547; ciocci, maria agnese /0000-0003-0002-5462; Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680; Matorras, Francisco/0000-0003-4295-5668; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Ferguson, Thomas/0000-0001-5822-3731; Benussi, Luigi/0000-0002-2363-8889; Russ, James/0000-0001-9856-9155; Dahms, Torsten/0000-0003-4274-5476; Grandi, Claudio/0000-0001-5998-3070; Chinellato, Jose Augusto/0000-0002-3240-6270; Montanari, Alessandro/0000-0003-2748-6373; Moon, Chang-Seong/0000-0001-8229-7829; Cerrada, Marcos/0000-0003-0112-1691; Scodellaro, Luca/0000-0002-4974-8330; Calvo Alamillo, Enrique/0000-0002-1100-2963; Tinoco Mendes, Andre David/0000-0001-5854-7699; Novaes, Sergio/0000-0003-0471-8549; Ligabue, Franco/0000-0002-1549-7107; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Dudko, Lev/0000-0002-4462-3192; Codispoti, Giuseppe/0000-0003-0217-7021; de Jesus Damiao, Dilson/0000-0002-3769-1680; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; FU Austrian Federal Ministry of Science and Research; Austrian Science Fund; Belgian Fonds de la Recherche Scientifique; Fonds voor Wetenschappelijk Onderzoek; CNPq; CAPES; FAPERJ; FAPESP; Bulgarian Ministry of Education and Science; CERN; Chinese Academy of Sciences; Ministry of Science and Technology; National Natural Science Foundation of China; Colombian Funding Agency (COLCIENCIAS); Croatian Ministry of Science, Education and Sport; Research Promotion Foundation, Cyprus; Ministry of Education and Research [SF0690030s09]; European Regional Development Fund, Estonia; Academy of Finland; Finnish Ministry of Education and Culture; Helsinki Institute of Physics; Institut National de Physique Nucleaire et de Physique des Particules / CNRS; Commissariat a l'Energie Atomique et aux Energies Alternatives / CEA, France; Bundesministerium fur Bildung und Forschung; Deutsche Forschungsgemeinschaft; Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; General Secretariat for Research and Technology, Greece; National Scientific Research Foundation; National Office for Research and Technology, Hungary; Department of Atomic Energy; Department of Science and Technology, India; Institute for Studies in Theoretical Physics and Mathematics, Iran; Science Foundation, Ireland; Istituto Nazionale di Fisica Nucleare, Italy; Korean Ministry of Education, Science and Technology; World Class University program of NRF, Republic of Korea; Lithuanian Academy of Sciences; CINVESTAV; CONACYT; SEP; UASLP-FAI; Ministry of Science and Innovation, New Zealand; Pakistan Atomic Energy Commission; Ministry of Science and Higher Education; National Science Centre, Poland; Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; Ministry of Education and Science of the Russian Federation; Federal Agency of Atomic Energy of the Russian Federation; Russian Academy of Sciences; Russian Foundation for Basic Research; Ministry of Education, Science and Technological Development of Serbia; Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio, Spain; ETH Board; ETH Zurich; PSI; SNF; UniZH; Canton Zurich; SER; National Science Council, Taipei; Thailand Center of Excellence in Physics; Institute for the Promotion of Teaching Science and Technology of Thailand; Special Task Force for Activating Research; National Science and Technology Development Agency of Thailand; Scientific and Technical Research Council of Turkey; Turkish Atomic Energy Authority; Science and Technology Facilities Council, U.K.; US Department of Energy; US National Science Foundation; Marie-Curie programme; European Research Council; EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of Czech Republic; Council of Science and Industrial Research, India; Compagnia di San Paolo (Torino); HOMING PLUS programme of Foundation for Polish Science; EU, Regional Development Fund; Thalis programme; Aristeia programme; EU-ESF; Greek NSRF FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centres and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: the Austrian Federal Ministry of Science and Research and the Austrian Science Fund; the Belgian Fonds de la Recherche Scientifique, and Fonds voor Wetenschappelijk Onderzoek; the Brazilian Funding Agencies (CNPq, CAPES, FAPERJ, and FAPESP); the Bulgarian Ministry of Education and Science; CERN; the Chinese Academy of Sciences, Ministry of Science and Technology, and National Natural Science Foundation of China; the Colombian Funding Agency (COLCIENCIAS); the Croatian Ministry of Science, Education and Sport; the Research Promotion Foundation, Cyprus; the Ministry of Education and Research, Recurrent financing contract SF0690030s09 and European Regional Development Fund, Estonia; the Academy of Finland, Finnish Ministry of Education and Culture, and Helsinki Institute of Physics; the Institut National de Physique Nucleaire et de Physique des Particules / CNRS, and Commissariat a l'Energie Atomique et aux Energies Alternatives / CEA, France; the Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft, and Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; the General Secretariat for Research and Technology, Greece; the National Scientific Research Foundation, and National Office for Research and Technology, Hungary; the Department of Atomic Energy and the Department of Science and Technology, India; the Institute for Studies in Theoretical Physics and Mathematics, Iran; the Science Foundation, Ireland; the Istituto Nazionale di Fisica Nucleare, Italy; the Korean Ministry of Education, Science and Technology and the World Class University program of NRF, Republic of Korea; the Lithuanian Academy of Sciences; the Mexican Funding Agencies (CINVESTAV, CONACYT, SEP, and UASLP-FAI); the Ministry of Science and Innovation, New Zealand; the Pakistan Atomic Energy Commission; the Ministry of Science and Higher Education and the National Science Centre, Poland; the Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; the Ministry of Education and Science of the Russian Federation, the Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences, and the Russian Foundation for Basic Research; the Ministry of Education, Science and Technological Development of Serbia; the Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio 2010, Spain; the Swiss Funding Agencies (ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER); the National Science Council, Taipei; the Thailand Center of Excellence in Physics, the Institute for the Promotion of Teaching Science and Technology of Thailand, Special Task Force for Activating Research and the National Science and Technology Development Agency of Thailand; the Scientific and Technical Research Council of Turkey, and Turkish Atomic Energy Authority; the Science and Technology Facilities Council, U.K.; the US Department of Energy, and the US National Science Foundation.; Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of Czech Republic; the Council of Science and Industrial Research, India; the Compagnia di San Paolo (Torino); the HOMING PLUS programme of Foundation for Polish Science, cofinanced by EU, Regional Development Fund; and the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF. NR 43 TC 11 Z9 11 U1 4 U2 103 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD OCT 24 PY 2013 IS 10 AR 167 DI 10.1007/JHEP10(2013)167 PG 45 WC Physics, Particles & Fields SC Physics GA 241TL UT WOS:000326190800001 ER PT J AU McKown, BG Ceriotti, M Womack, CC Kamarchik, E Butler, LJ Bowman, JM AF McKown, Benjamin G. Ceriotti, Michele Womack, Caroline C. Kamarchik, Eugene Butler, Laurie J. Bowman, Joel M. TI Effects of High Angular Momentum on the Unimolecular Dissociation of CD2CD2OH: Theory and Comparisons with Experiment SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID POTENTIAL-ENERGY SURFACE; PLUS VINYL PRODUCTS; ELASTIC BAND METHOD; AB-INITIO; DIFFUSION MAPS; SKETCH-MAP; 193 NM; RADICAL INTERMEDIATE; MOLECULAR-DYNAMICS; RATE CONSTANTS AB This paper explores the dynamics of a highly rotationally and vibrationally excited radical, CD2CD2OH. The radical is produced from the 193 nm photodissociation of 2-bromoethanol-d(4), so it is imparted with high angular momentum and high vibrational energy and subsequently dissociates to several product channels. This paper focuses on characterizing its angular momentum and modeling its effect on the product channels, including the HOD + vinyl-d(3) product channel resulting from a frustrated dissociation of the radical originally en route to OH + ethene-d(4) that instead results in D atom abstraction. Our impulsive model of the initial photodissociation shows that, for some cases, upward of 200 au of angular momentum is imparted, which greatly affects the dynamics of the competing product channels. Using a permutationally invariant potential energy surface and quasiclassical trajectories, we simulated the dissociation dynamics of CD2CD2OH and compared these results to those of Kamarchik et al. (J. Phys. Chem. Lett. 2010, 1, 3058-3065), who studied the dynamics of CH2CH2OH with zero angular momentum. We found that the recoil translational energy distribution for radicals that dissociated to OH + C2D4 matched experiment closely only when high angular momentum of the initial radical was explicitly included in the trajectory calculations. Similarly, the rate constant for dissociation changes when rotational energy was added to the vibrational energy in the initial conditions. Lastly, we applied the sketch-map dimensionality reduction technique to analyze mechanistic information leading to the vinyl + water product channel. Projecting the ab initio intrinsic reaction coordinates onto the lower dimensional space identified with sketch map offers new insight into the dynamics when one looks at the simulated trajectories in the lower dimensional space. Further analysis shows that the transition path resembles a frustrated dissociation of the OH + ethene radical adduct, followed instead by branching to vinyl + water when the leaving OH group encounters a nearby D atom on the ethene moiety. This characterization is in accord with the one made previously. We show that the transition path bifurcation between the two similar channels occurs at carbon - oxygen distances and oxygen-abstracted deuterium distances of 2-2.5 angstrom controlled by the C-O-D bond angle with large angles preferentially branching to the water plus vinyl product state. The experimental branching ratios were not reproduced by theory, however, due partly to the insufficient quality of the fitted potential surface. We also have evidence of a minor product channel, HD + vinoxy-d(3), from our molecular dynamics simulations that allows us to assign the HD signal in prior experimental work. C1 [McKown, Benjamin G.; Womack, Caroline C.; Butler, Laurie J.] Univ Chicago, Dept Chem, Chicago, IL 60637 USA. [McKown, Benjamin G.; Womack, Caroline C.; Butler, Laurie J.] Univ Chicago, James Franck Inst, Chicago, IL 60637 USA. [Ceriotti, Michele] Ecole Polytech Fed Lausanne, Inst Mat, CH-1015 Lausanne, Switzerland. [Kamarchik, Eugene] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA. [Bowman, Joel M.] Emory Clin, Dept Chem, Cherry L Emerson Ctr Sci Computat, Atlanta, GA 30322 USA. RP Butler, LJ (reprint author), Univ Chicago, Dept Chem, 5735 S Ellis Ave, Chicago, IL 60637 USA. EM l-butler@uchicago.edu RI Ceriotti, Michele/C-2393-2009; Womack, Caroline/C-7818-2016 OI Ceriotti, Michele/0000-0003-2571-2832; FU Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy [DE-FG02-92ER1430S, DE-FG02-97ER14782, DE-AC04-94-AL85000]; EU Marie Curie IEF [PIEF-GA-2010-272402] FX This work was supported by the Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy, under Grants DE-FG02-92ER1430S (L.J.B.), DE-FG02-97ER14782 (J.M.B), and DE-AC04-94-AL85000 (E.K) and by the EU Marie Curie IEF No. PIEF-GA-2010-272402 (M.C.). NR 46 TC 11 Z9 11 U1 0 U2 21 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 EI 1520-5215 J9 J PHYS CHEM A JI J. Phys. Chem. A PD OCT 24 PY 2013 VL 117 IS 42 BP 10951 EP 10963 DI 10.1021/jp407913t PG 13 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 242RM UT WOS:000326259700014 PM 24124756 ER PT J AU Shen, TY Qi, XH Nellas, RB AF Shen, Tongye Qi, Xianghong Nellas, Ricky B. TI Nucleation Dynamics of Active Particles SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID AZOSPIRILLUM-BRASILENSE; GLASSES; MECHANICS; PATHWAY AB We present a model of a collection of active and adhesive Brownian particles that are capable of aggregation. Besides the mechanical interaction between particles, a simple active dynamics term (motility) is included to provide an active movement. At a given instant, each particle is either in an active (swim) or unanimated (stop) state, which is controlled by a random process. The model includes important features that are inspired by the phenomenon of biological cell-cell association. One feature is the mean motility that is related to the percentage of the particle being active and the maximum swimming speed. Another feature is the stochastic nature of switching between the swim and stop state. We explored how these key features affect the nucleation dynamics and the stability of the aggregates using simulations. Interestingly, particles can change their collective behavior by solely altering the frequency of switching between the swim and stop state while keeping the mean motility unchanged. These results provide insight into how motor-driven forces can be utilized by active biological systems to modulate the single-to-cluster transition efficiently. A dimensionless parameter is also proposed to measure the overall strength of the nonequilibrium effect on active particles. C1 [Shen, Tongye; Qi, Xianghong; Nellas, Ricky B.] Univ Tennessee, Dept Biochem Cellular & Mol Biol, Knoxville, TN 37996 USA. [Shen, Tongye; Qi, Xianghong; Nellas, Ricky B.] Oak Ridge Natl Lab, UT ORNL Ctr Mol Biophys, Oak Ridge, TN 37830 USA. RP Shen, TY (reprint author), Univ Tennessee, Dept Biochem Cellular & Mol Biol, Knoxville, TN 37996 USA. EM tshen@utk.edu RI Shen, Tongye/A-9718-2008 OI Shen, Tongye/0000-0003-1495-3104 NR 30 TC 1 Z9 1 U1 1 U2 9 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD OCT 24 PY 2013 VL 117 IS 42 BP 12844 EP 12849 DI 10.1021/jp402024s PG 6 WC Chemistry, Physical SC Chemistry GA 242RN UT WOS:000326259800020 PM 23819710 ER PT J AU Frauenfelder, H Young, RD Fenimore, PW AF Frauenfelder, Hans Young, Robert D. Fenimore, Paul W. TI Dynamics and the Free-Energy Landscape of Proteins, Explored with the Mossbauer Effect and Quasi-Elastic Neutron Scattering SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID MACROMOLECULAR SYSTEMS; RESONANCE ABSORPTION; GAMMA-RESONANCE; FLUCTUATIONS; MYOGLOBIN; SPECTROSCOPY; TEMPERATURE; CRYSTALS; MOTIONS; TRANSITION AB The Mossbauer effect and quasi-elastic neutron scattering (QENS) from hydrated proteins yield sharp elastic lines that are accompanied by broad wings. Conventionally, the elastic line and the broad wings are treated as separate phenomena. We show that there is no separation; the entire spectrum consists of Lorentzians with the natural line width. In protein crystals, the shifts of the individual lines from the elastic center above about 150 K are caused by beta fluctuations in the hydration shell. Vibrations cause shifts in the entire temperature range but are best seen below about 150 K. We construct a microscopic model for the dynamics that is based on a random walk of the proteins in their free-energy landscape. The model yields approximate values for the steps in the energy landscape. Remarkably, the quantum electrodynamic concept of gamma rays is needed to justify the model. C1 [Frauenfelder, Hans; Fenimore, Paul W.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Young, Robert D.] Arizona State Univ, Ctr Theoret Biol Phys, Tempe, AZ 85287 USA. RP Fenimore, PW (reprint author), Los Alamos Natl Lab, T6, Los Alamos, NM 87545 USA. EM paulf@lanl.gov FU Department of Energy [DE-ACS206NA25396] FX The work was supported by Department of Energy Contract DE-ACS206NA25396. Illuminating discussions with Ben McMahon helped us to understand the role of vibrations. Without help from Marlan Scully and Dmitri Voronine, who explained the true nature of light to us, we would still wonder if our model is based on solid ground. NR 49 TC 6 Z9 6 U1 1 U2 27 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 EI 1520-5207 J9 J PHYS CHEM B JI J. Phys. Chem. B PD OCT 24 PY 2013 VL 117 IS 42 BP 13301 EP 13307 DI 10.1021/jp403832n PG 7 WC Chemistry, Physical SC Chemistry GA 242RN UT WOS:000326259800065 PM 23962200 ER PT J AU Lee, CH Orloff, ND Birol, T Zhu, Y Goian, V Rocas, E Haislmaier, R Vlahos, E Mundy, JA Kourkoutis, LF Nie, YF Biegalski, MD Zhang, JS Bernhagen, M Benedek, NA Kim, Y Brock, JD Uecker, R Xi, XX Gopalan, V Nuzhnyy, D Kamba, S Muller, DA Takeuchi, I Booth, JC Fennie, CJ Schlom, DG AF Lee, Che-Hui Orloff, Nathan D. Birol, Turan Zhu, Ye Goian, Veronica Rocas, Eduard Haislmaier, Ryan Vlahos, Eftihia Mundy, Julia A. Kourkoutis, Lena F. Nie, Yuefeng Biegalski, Michael D. Zhang, Jingshu Bernhagen, Margitta Benedek, Nicole A. Kim, Yongsam Brock, Joel D. Uecker, Reinhard Xi, X. X. Gopalan, Venkatraman Nuzhnyy, Dmitry Kamba, Stanislav Muller, David A. Takeuchi, Ichiro Booth, James C. Fennie, Craig J. Schlom, Darrell G. TI Exploiting dimensionality and defect mitigation to create tunable microwave dielectrics SO NATURE LA English DT Article ID NETWORK-ANALYZER CALIBRATION; MOLECULAR-BEAM EPITAXY; THIN-FILMS; DEPENDENCE; TITANIUM; DEVICES; SRTIO3; OXIDES; FERROELECTRICITY; DISPERSION AB The miniaturization and integration of frequency-agile microwave circuits-relevant to electronically tunable filters, antennas, resonators and phase shifters-with microelectronics offers tantalizing device possibilities, yet requires thin films whose dielectric constant at gigahertz frequencies can be tuned by applying a quasi-static electric field(1). Appropriate systems such as BaxSr1-xTiO3 have a paraelectric-ferroelectric transition just below ambient temperature, providing high tunability(1-3). Unfortunately, such films suffer significant losses arising from defects. Recognizing that progress is stymied by dielectric loss, we start with a system with exceptionally low loss-Srn+1TinO3n+1 phases(4,5)-in which (SrO)(2) crystallographic shear(6,7) planes provide an alternative to the formation of point defects for accommodating non-stoichiometry(8,9). Here we report the experimental realization of a highly tunable ground state arising from the emergence of a local ferroelectric instability(10) in biaxially strained Srn+1TinO3n+1 phases with n >= 3 at frequencies up to 125 GHz. In contrast to traditional methods of modifying ferroelectrics-doping(1-3,11,12) or strain(13-16)-in this unique system an increase in the separation between the (SrO)(2) planes, which can be achieved by changing n, bolsters the local ferroelectric instability. This new control parameter, n, can be exploited to achieve a figure of merit at room temperature that rivals all known tunable microwave dielectrics(3). C1 [Lee, Che-Hui; Nie, Yuefeng; Zhang, Jingshu; Schlom, Darrell G.] Cornell Univ, Dept Mat Sci & Engn, Ithaca, NY 14853 USA. [Lee, Che-Hui; Haislmaier, Ryan; Vlahos, Eftihia; Gopalan, Venkatraman] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. [Orloff, Nathan D.; Booth, James C.] NIST, Boulder, CO 80305 USA. [Orloff, Nathan D.] Univ Maryland, Dept Phys, College Pk, MD 20742 USA. [Birol, Turan; Zhu, Ye; Mundy, Julia A.; Kourkoutis, Lena F.; Kim, Yongsam; Brock, Joel D.; Muller, David A.; Fennie, Craig J.] Cornell Univ, Sch Appl & Engn Phys, Ithaca, NY 14853 USA. [Goian, Veronica; Nuzhnyy, Dmitry; Kamba, Stanislav] Inst Phys ASCR, Prague 18221 8, Czech Republic. [Rocas, Eduard] Univ Politecn Cataluna, Dept Signal Theory & Commun, ES-08034 Barcelona, Spain. [Kourkoutis, Lena F.; Muller, David A.; Schlom, Darrell G.] Kavli Inst Cornell Nanoscale Sci, Ithaca, NY 14853 USA. [Biegalski, Michael D.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Bernhagen, Margitta; Uecker, Reinhard] Leibniz Inst Crystal Growth, D-12489 Berlin, Germany. [Benedek, Nicole A.] Univ Texas Austin, Mat Sci & Engn Program, Austin, TX 78712 USA. [Xi, X. X.] Temple Univ, Dept Phys, Philadelphia, PA 19122 USA. [Takeuchi, Ichiro] Univ Maryland, Dept Mat Sci & Engn, College Pk, MD 20742 USA. RP Schlom, DG (reprint author), Cornell Univ, Dept Mat Sci & Engn, Ithaca, NY 14853 USA. EM schlom@cornell.edu RI Nie, Yuefeng/A-1595-2013; Birol, Turan/D-1948-2012; Kamba, Stanislav/G-5332-2014; Nie, Yuefeng/L-8071-2013; Zhu, Ye/A-1844-2011; Goian, Veronica/G-6154-2014; Nuzhnyy, Dmitry/G-6661-2014; OI Nie, Yuefeng/0000-0002-3449-5393; Birol, Turan/0000-0001-5174-3320; Kamba, Stanislav/0000-0003-4699-869X; Nie, Yuefeng/0000-0002-3449-5393; Zhu, Ye/0000-0002-5217-493X; Goian, Veronica/0000-0002-7971-2224; Orloff, Nathan/0000-0001-5391-4699; Muller, David/0000-0003-4129-0473; Kourkoutis, Lena/0000-0002-1303-1362 FU Army Research Office (ARO) [W911NF-09-1-0415, W911NF-12-1-0437, W911NF-10-1-0345]; National Science Foundation (NSF) through Materials Research Science and Engineering Centers (MRSEC) [DMR-0820404, DMR-1120296]; Czech Science Foundation [P204/12/1163]; Czech Ministry of Education, Youth and Sports [LD12026]; Spanish Government; European Union [EUI-ENIAC-2011-4349, EUI-ENIAC 2010-04252]; NSF [DMR-0820404]; National Defense Science & Engineering Graduate Fellowship; Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy; National Science Foundation [ECCS-0335765]; NSF MRSEC programme [DMR 1120296, NSF IMR-0417392] FX We acknowledge discussions with S. Trolier-McKinstry and C. A. Randall. Research was supported by Army Research Office (ARO) grants W911NF-09-1-0415 (for C.-H. L., Y. Z., J. A. M. and D. A. M.), W911NF-12-1-0437 (for Y. N., J. Z. and D. G. S.) and W911NF-10-1-0345 (for T. B., N. A. B. and C. J. F.); by the National Science Foundation (NSF) through Materials Research Science and Engineering Centers (MRSEC) grants DMR-0820404 (for R. H., E. V., X. X. X. and V. G.) and DMR-1120296 (for Y. K., J. D. B. and L. F. K.); by the Czech Science Foundation Project no. P204/12/1163 and the Czech Ministry of Education, Youth and Sports project LD12026 (for V. G., D. N. and S. K.); and by the Spanish Government and the European Union through grants EUI-ENIAC-2011-4349 and EUI-ENIAC 2010-04252 (for E. R.). C.-H. L. acknowledges stipend support from NSF grant DMR-0820404. J. A. M. acknowledges financial support from a National Defense Science & Engineering Graduate Fellowship. The dielectric and ferroelectric measurements in Fig. 3c were conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. This work was performed in part at the Cornell NanoScale Factory, a member of the National Nanotechnology Infrastructure Network, which is supported by the National Science Foundation (grant ECCS-0335765). This work made use of the electron microscopy facility of the Cornell Center for Materials Research (CCMR) with support fromthe NSF MRSEC programme (DMR 1120296) and NSF IMR-0417392. NR 47 TC 64 Z9 64 U1 23 U2 247 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD OCT 24 PY 2013 VL 502 IS 7472 BP 532 EP + DI 10.1038/nature12582 PG 18 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 238YN UT WOS:000325988400050 PM 24132232 ER PT J AU Jarenwattananon, NN Gloggler, S Otto, T Melkonian, A Morris, W Burt, SR Yaghi, OM Bouchard, LS AF Jarenwattananon, Nanette N. Gloeggler, Stefan Otto, Trenton Melkonian, Arek Morris, William Burt, Scott R. Yaghi, Omar M. Bouchard, Louis-S. TI Thermal maps of gases in heterogeneous reactions SO NATURE LA English DT Article ID METAL-ORGANIC FRAMEWORKS; PARA-HYDROGEN; INDUCED POLARIZATION; MAGNETIC-RESONANCE; PARAHYDROGEN; CATALYSTS AB More than 85 per cent of all chemical industry products are made using catalysts(1,2), the overwhelming majority of which are heterogeneous catalysts(2) that function at the gas-solid interface(3). Consequently, much effort is invested in optimizing the design of catalytic reactors, usually by modelling(4) the coupling between heat transfer, fluid dynamics and surface reactionkinetics. The complexity involved requires a calibration of model approximations against experimental observations(5,6), with temperature maps being particularly valuable because temperature control is often essential for optimal operation and because temperature gradients contain information about the energetics of a reaction. However, it is challenging to probe the behaviour of a gas inside a reactor without disturbing its flow, particularly when trying also to map the physical parameters and gradients that dictate heat and mass flow and catalytic efficiency(1-9). Although optical techniques(10-12) and sensors(13,14) have been used for that purpose, the former perform poorly in opaque media and the latter perturb the flow. NMR thermometry can measure temperature non-invasively, but traditional approaches applied to gases produce signals that depend only weakly on temperature(15,16) are rapidly attenuated by diffusion(16,17) or require contrast agents(18) that may interfere with reactions. Here we present a new NMR thermometry technique that circumvents these problems by exploiting the inverse relationship between NMR line-widths and temperature caused by motional averaging in a weak magnetic field gradient. We demonstrate the concept by non-invasively mapping gas temperatures during the hydrogenation of propylene in reactors packed with metal nanoparticles and metal-organic framework catalysts, with measurement errors of less than four per cent of the absolute temperature. These results establish our technique as a non-invasive tool for locating hot and cold spots in catalyst-packed gas-solid reactors, with unprecedented capabilities for testing the approximations used in reactor modelling. C1 [Jarenwattananon, Nanette N.; Gloeggler, Stefan; Otto, Trenton; Melkonian, Arek; Morris, William; Yaghi, Omar M.; Bouchard, Louis-S.] Univ Calif Los Angeles, Dept Chem & Biochem, Los Angeles, CA 90095 USA. [Burt, Scott R.] Brigham Young Univ, Dept Chem & Biochem, Provo, UT 84602 USA. [Yaghi, Omar M.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Yaghi, Omar M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Yaghi, Omar M.] NanoCentury KAIST Inst, Taejon 305701, South Korea. [Yaghi, Omar M.] World Class Univ, Grad Sch Energy Environm Water & Sustainabil, Taejon 305701, South Korea. [Bouchard, Louis-S.] Univ Calif Los Angeles, Calif NanoSyst Inst, Los Angeles, CA 90095 USA. [Bouchard, Louis-S.] Univ Calif Los Angeles, Dept Bioengn, Los Angeles, CA 90095 USA. RP Bouchard, LS (reprint author), Univ Calif Los Angeles, Dept Chem & Biochem, 607 Charles E Young Dr East, Los Angeles, CA 90095 USA. EM bouchard@chem.ucla.edu OI Yaghi, Omar/0000-0002-5611-3325 FU Dreyfus New Faculty Award; Beckman Young Investigator Award; US NSF [CHE-1153159]; BASF, Germany (synthesis); US DOE FX We thank J. Reimer, C. T. Campbell, W. S. Warren, I. Oppenheim and R. Bruinsma for discussions; N. K. Garg, C. T. Campbell, W. Gelbart and C. Knobler for reading the manuscript; M. T. Yeung for technical help with MATLAB; and J. Brown and R. Sharma for assistance with chemical synthesis. This work was funded by a Dreyfus New Faculty Award (L.-S.B.); a Beckman Young Investigator Award (L.-S.B.); US NSF CHE-1153159 (L.-S.B., O.M.Y.); BASF, Germany (synthesis); and the US DOE (O.M.Y.; porosity measurements). NR 30 TC 19 Z9 19 U1 12 U2 190 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD OCT 24 PY 2013 VL 502 IS 7472 BP 537 EP + DI 10.1038/nature12568 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 238YN UT WOS:000325988400051 PM 24153305 ER PT J AU Wang, CJ Han, Y Walen, H Russell, SM Thiel, PA Evans, JW AF Wang, Chi-Jen Han, Yong Walen, Holly Russell, Selena M. Thiel, Patricia A. Evans, James W. TI Analytic formulations for one-dimensional decay of rectangular homoepitaxial islands during coarsening on anisotropic fcc (110) surfaces SO PHYSICAL REVIEW B LA English DT Article ID EPITAXIAL-GROWTH; METAL-SURFACES; KINETIC-MODEL; MONTE-CARLO; STEP; NANOSTRUCTURES; AG(110); TRANSITION AB Submonolayer homoepitaxial fcc (110) systems display behavior reflecting strong anisotropy at lower temperatures, including one-dimensional decay during Ostwald ripening of rectangular islands maintaining constant width in the < 001 > direction. To appropriately describe this behavior, we first develop a refined continuum Burton-Cabrera-Frank formalism, which accounts for a lack of equilibration of island shape and importantly also for inhibited incorporation of adatoms at almost-faceted <(1) over bar 10 > island edges through effective kinetic coefficients. This formalism is shown to describe accurately the adatom diffusion fluxes between islands and thus island evolution for a complex experimental island configuration, as confirmed by matching results from realistic atomistic simulations for this configuration. This approach also elucidates basic dependencies of flux on island geometry and temperature. Second, a further refinement is presented incorporating separate terrace and edge adatom density fields either in a continuum setting or alternatively in a spatially discrete diffusion equation setting. The second approach allows more flexibility and accuracy in accounting for edge-diffusion kinetics including corner rounding, a lack of equilibration of the edge adatom density at <(1) over bar 10 > island edges, and the effect of rare kinks on <(1) over bar 10 > island edges. Significantly, it suggests facile two-way corner rounding at the island periphery during island decay, contrasting the previous picture. C1 [Wang, Chi-Jen; Evans, James W.] Iowa State Univ, Dept Math, Ames, IA 50011 USA. [Han, Yong; Evans, James W.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Walen, Holly; Russell, Selena M.; Thiel, Patricia A.] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. [Thiel, Patricia A.; Evans, James W.] Iowa State Univ, US Dept Energy, Ames Lab, Ames, IA 50011 USA. RP Wang, CJ (reprint author), Iowa State Univ, Dept Math, Ames, IA 50011 USA. EM yong@ameslab.gov RI Russell, Selena/C-6896-2009; Walen, Holly/O-6462-2014 OI Russell, Selena/0000-0001-7196-6409; FU NSF [CHE-1111500]; USDOE by Iowa State University [DE-AC02-07CH11358] FX This work was supported by NSF Grant No. CHE-1111500. It was performed at Ames Laboratory, which is operated for the USDOE by Iowa State University under Contract No. DE-AC02-07CH11358. We thank Dr. Anthony R. Layson for providing some of the STM data. NR 27 TC 3 Z9 3 U1 1 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 24 PY 2013 VL 88 IS 15 AR 155434 DI 10.1103/PhysRevB.88.155434 PG 10 WC Physics, Condensed Matter SC Physics GA 240JV UT WOS:000326092900002 ER PT J AU Catterall, S Giedt, J Joseph, A AF Catterall, Simon Giedt, Joel Joseph, Anosh TI Twisted supersymmetries in lattice N=4 super Yang-Mills theory SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Lattice Quantum Field Theory; Supersymmetric gauge theory; Extended Supersymmetry; Topological Field Theories AB Recently it has been shown how a topologically twisted version of N = 4 super Yang-Mills may be discretized in such a way as to preserve one scalar supersymmetry at nonzero lattice spacing. The remaining fifteen supersymmetries are broken by terms of O(a) where a is the lattice spacing. One would like to know whether these remaining supersymmetries are regained in the continuum limit a -> 0 and, if not, how much tuning of the couplings in the lattice action is required. In this paper we derive the form of these additional twisted supersymmetries by combining a set of discrete R-symmetries of the continuum theory with the action of the scalar supersymmetry. We then argue that restoration of rotational symmetry in the continuum limit of the lattice theory likely implies restoration of R-symmetry and hence should lead to an automatic enhancement to the full N = 4 supersymmetry without further fine-tuning. C1 [Catterall, Simon] Syracuse Univ, Dept Phys, Syracuse, NY 13244 USA. [Giedt, Joel] Rensselaer Polytech Inst, Dept Phys Appl Phys & Astron, Troy, NY 12065 USA. [Joseph, Anosh] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Catterall, S (reprint author), Syracuse Univ, Dept Phys, Syracuse, NY 13244 USA. EM smc@physics.syr.edu; giedtj@rpi.edu; anoshjoseph@gmail.com RI Joseph, Anosh/F-9283-2012; OI Joseph, Anosh/0000-0003-4288-8207; Catterall, Simon/0000-0003-2735-2682 FU U.S. Department of Energy [DE-FG02-85ER40237, DE-FG02-08ER41575]; LDRD program at the Los Alamos National Laboratory; National Science Foundation [PHY-1066293] FX This work was supported in part by the U.S. Department of Energy grant under Contract No. DE-FG02-85ER40237 (SC) and DE-FG02-08ER41575 (JG) and the LDRD program at the Los Alamos National Laboratory (AJ). SC and JG also acknowledge the hospitality of the Aspen Center for Physics, which is supported by the National Science Foundation Grant No. PHY-1066293, where some of this work was conducted. NR 35 TC 9 Z9 9 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD OCT 24 PY 2013 IS 10 AR 166 DI 10.1007/JHEP10(2013)166 PG 24 WC Physics, Particles & Fields SC Physics GA 240GT UT WOS:000326083800002 ER PT J AU Biersack, HJ Ezziddin, S Knapp, FF AF Biersack, Hans-Juergen Ezziddin, Samer Knapp, Furn F. TI Radium-223 in Prostate Cancer SO NEW ENGLAND JOURNAL OF MEDICINE LA English DT Letter ID PALLIATION; SURVIVAL; THERAPY AB To the Editor: In their editorial on the use of radium-223 for the treatment of bone metastases in prostate cancer, Vapiwala and Glatstein (July 18 issue)(1) provide an overview of the benefits of alpha-emitting radioisotopes. They focus on the results reported in the same issue of the Journal by Parker et al.,(2) who describe the association between the use of radium-223 dichloride and an observed increase in survival, as compared with placebo. In both the article and the editorial, the authors suggest that current radiopharmaceutical agents for bone pain palliation do not prolong survival, with the editorialists stating that the ... C1 [Biersack, Hans-Juergen; Ezziddin, Samer] Univ Hosp Bonn, Bonn, Germany. [Knapp, Furn F.] Oak Ridge Natl Lab, Oak Ridge, TN USA. RP Biersack, HJ (reprint author), Univ Hosp Bonn, Bonn, Germany. EM hans-juergen.biersack@ukb.uni-bonn.de NR 6 TC 1 Z9 1 U1 0 U2 5 PU MASSACHUSETTS MEDICAL SOC PI WALTHAM PA WALTHAM WOODS CENTER, 860 WINTER ST,, WALTHAM, MA 02451-1413 USA SN 0028-4793 EI 1533-4406 J9 NEW ENGL J MED JI N. Engl. J. Med. PD OCT 24 PY 2013 VL 369 IS 17 BP 1659 EP 1659 DI 10.1056/NEJMc1310231 PG 1 WC Medicine, General & Internal SC General & Internal Medicine GA 239MZ UT WOS:000326031100017 PM 24152266 ER PT J AU Kogan, VG AF Kogan, V. G. TI Elastic contribution to interaction of vortices in uniaxial superconductors SO PHYSICAL REVIEW B LA English DT Article AB The stress caused by vortices in tetragonal superconductors contributes to the intervortex interaction which depends on vortex orientation within the crystal, on elastic moduli, and is attractive within certain angular regions even in fields along the c crystal axis. For sufficiently strong stress dependence of the critical temperature, this contribution may result in distortions of the hexagonal vortex lattice for H parallel to c. In small fields it leads to formation of a square vortex lattice with a fixed H independent spacing. This should be seen in the magnetization M(H) as a discontinuous jump of magnetization at the transition from the Meissner to mixed states. C1 [Kogan, V. G.] Iowa State Univ, US DOE, Ames Lab, Ames, IA 50011 USA. [Kogan, V. G.] Iowa State Univ, Dept Phys, Ames, IA 50011 USA. RP Kogan, VG (reprint author), Iowa State Univ, US DOE, Ames Lab, Ames, IA 50011 USA. EM kogan@ameslab.gov FU Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-AC02-07CH11358] FX The author is grateful to J. Clem, S. Bud'ko, R. Prozorov, and M. Tanatar for helpful discussions. The Ames Laboratory is supported by the Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Contract No. DE-AC02-07CH11358. NR 13 TC 1 Z9 1 U1 0 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 24 PY 2013 VL 88 IS 14 AR 144514 DI 10.1103/PhysRevB.88.144514 PG 5 WC Physics, Condensed Matter SC Physics GA 240JU UT WOS:000326092800003 ER PT J AU Mann, GW Calley, PC Joshi, HJ Heazlewood, JL AF Mann, Gregory W. Calley, Paul C. Joshi, Hiren J. Heazlewood, Joshua L. TI MASCP gator: an overview of the Arabidopsis proteomic aggregation portal SO FRONTIERS IN PLANT SCIENCE LA English DT Review DE proteomics; Arabidopsis; mass spectrometry; database; protein modifications; single nucleotide; polymorphisms ID INFORMATION RESOURCE TAIR; N-TERMINAL MODIFICATIONS; PLANT-MITOCHONDRIA; PROTEIN-PHOSPHORYLATION; AFFINITY PURIFICATION; CHLOROPLAST PROTEOME; SORTING SIGNALS; S-NITROSYLATION; THALIANA; DATABASE AB A key challenge in the area of bioinformatics in the coming decades is the ability to manage the wealth of information that is being generated from the variety of high throughput methodologies currently being undertaken in laboratories across the world. While these approaches have made available large volumes of data to the research community, less attention has been given to the problem of how to intuitively present the data to enable greater biological insights. Recently, an attempt was made to tackle this problem in the area of Arabidopsis proteomics. The model plant has been the target of countless proteomics surveys producing an exhaustive array of data and online repositories. The MASCP Gator is an aggregation portal for proteomic data currently being produced by the community and unites a large collection of specialized resources to a single portal (http://gator.masc-proteomics.org/). Here we describe the latest additions, upgrades and features to this resource further expanding its role into protein modifications and genome sequence variations. C1 [Mann, Gregory W.; Calley, Paul C.; Heazlewood, Joshua L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint BioEnergy Inst, Berkeley, CA 94720 USA. [Mann, Gregory W.; Calley, Paul C.; Heazlewood, Joshua L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Joshi, Hiren J.] Univ Copenhagen, Copenhagen Ctr Glyc, Inst Cellular & Mol Med, Copenhagen, Denmark. RP Heazlewood, JL (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint BioEnergy Inst, 1 Cyclotron Rd MS 978-4466, Berkeley, CA 94720 USA. EM jlheazlewood@lbl.gov RI Heazlewood, Joshua/A-2554-2008 OI Heazlewood, Joshua/0000-0002-2080-3826 FU Joint BioEnergy Institute; Office of Science, Office of Biological and Environmental Research, of the U.S. Department of Energy [DE-ACO2-05CH11231] FX The MASCP Gator was created with the support of members of the Arabidopsis proteomics community who assisted in the development of database specific services to enable data exchange. This work was conducted by the Joint BioEnergy Institute and is supported by the Office of Science, Office of Biological and Environmental Research, of the U.S. Department of Energy under Contract No. DE-ACO2-05CH11231. NR 52 TC 6 Z9 6 U1 0 U2 5 PU FRONTIERS RESEARCH FOUNDATION PI LAUSANNE PA PO BOX 110, LAUSANNE, 1015, SWITZERLAND SN 1664-462X J9 FRONT PLANT SCI JI Front. Plant Sci. PD OCT 23 PY 2013 VL 4 AR 411 DI 10.3389/fpls.2013.00411 PG 6 WC Plant Sciences SC Plant Sciences GA AA8XV UT WOS:000331379200001 PM 24167507 ER PT J AU So, MC Jin, S Son, HJ Wiederrecht, GP Farha, OK Hupp, JT AF So, Monica C. Jin, Shengye Son, Ho-Jin Wiederrecht, Gary P. Farha, Omar K. Hupp, Joseph T. TI Layer-by-Layer Fabrication of Oriented Porous Thin Films Based on Porphyrin-Containing Metal-Organic Frameworks SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID CHARGE MOBILITY; ENERGY-TRANSFER; GROWTH AB We report the synthesis and characterization of two thin films (DA-MOF and L2-MOF) of porphyrin-based MOFs on functionalized surfaces using a layer-by-layer (LbL) approach. Profilometry measurements confirm that the film thickness increases systematically with number of growth cycles. Polarization excitation and fluorescence measurements indicate that the porphyrin units are preferentially oriented, while X-ray reflectivity scans point to periodic ordering. Ellipsometry measurements show that the films are highly porous. Since there are currently few methods capable of yielding microporous MOFs containing accessible free-base porphyrins, it is noteworthy that the LbL growth permits direct MOF incorporation of unmetalated porphyrins. Long-range energy transfer is demonstrated for both MOF films. The findings offer useful insights for subsequent fabrication of MOF-based solar energy conversion devices. C1 [So, Monica C.; Son, Ho-Jin; Farha, Omar K.; Hupp, Joseph T.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Jin, Shengye; Wiederrecht, Gary P.] Argonne Natl Lab, Nanosci & Technol Div, Argonne, IL 60439 USA. RP Wiederrecht, GP (reprint author), Argonne Natl Lab, Nanosci & Technol Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM wiederrecht@anl.gov; o-farha@northwestern.edu; j-hupp@northwestern.edu RI Farha, Omar/B-5512-2014 OI Farha, Omar/0000-0002-9904-9845 FU Department of Defense through the National Defense Science & Engineering Graduate Fellowship (NDSEG) Program; Northwestern University; U.S. Dept. of Energy, Office of Science, Office of Basic Energy Sciences [DE-FG02-87ER13808, DE-SC0001059, DE-AC02- 06CH11357]; MRSEC program of the NSF at the NU Materials Research Center [DMR-1121262] FX We thank A. Smeigh, S. Kelwaramani, and O. Shekhah for helpful discussions. M.C.S. acknowledges support from the Department of Defense through the National Defense Science & Engineering Graduate Fellowship (NDSEG) Program. J.T.H. gratefully acknowledges support from Northwestern University and from the U.S. Dept. of Energy, Office of Science, Office of Basic Energy Sciences (grant no. DE-FG02-87ER13808). S.J., who contributed polarized fluorescence measurements, was supported at the Nanoscience & Technology Division by the ANSER Center, an Energy Frontier Research Center funded by the U.S. Dept. of Energy, Office of Science, Office of Basic Energy Sciences, under award no. DE-SC0001059. Use of Center of Nanoscale Materials is funded by the U.S. Dept. of Energy, Office of Science, Office of Basic Energy Sciences through contract no. DE-AC02- 06CH11357. We made use of the J.B. Cohen X-Ray Diffraction Facility supported by the MRSEC program of the NSF (DMR-1121262) at the NU Materials Research Center. NR 29 TC 98 Z9 99 U1 26 U2 268 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 EI 1520-5126 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD OCT 23 PY 2013 VL 135 IS 42 BP 15698 EP 15701 DI 10.1021/ja4078705 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA 242CV UT WOS:000326215900009 PM 24127847 ER PT J AU Wood, BC Schwegler, E Choi, WI Ogitsu, T AF Wood, Brandon C. Schwegler, Eric Choi, Woon Ih Ogitsu, Tadashi TI Hydrogen-Bond Dynamics of Water at the Interface with InP/GaP(001) and the Implications for Photoelectrochemistry SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID DENSITY-FUNCTIONAL THEORY; GROUP METAL CATALYST; TIO2 ANATASE 101; MOLECULAR-DYNAMICS; PROTON CONDUCTION; INP PHOTOCATHODES; INDIUM-PHOSPHIDE; SILICA GLASSES; 001 SURFACES; SOLAR-CELLS AB We investigate the structure, topology, and dynamics of liquid water at the interface with natively hydroxylated (001) surfaces of InP and GaP photoelectrodes. Using ab initio molecular dynamics simulations, we show that contact with the semiconductor surface enhances the water hydrogen-bond strength at the interface. This leads to the formation of an ice-like structure, within which dynamically driven water dissociation and local proton hopping are amplified. Nevertheless, the structurally similar and isovalent InP and GaP surfaces generate qualitatively different interfacial water dynamics. This can be traced to slightly more covalent-like character in the binding of surface adsorbates to GaP, which results in a more rigid hydrogen-bond network that limits the explored topological phase space. As a consequence, local proton hopping can give rise to long-range surface proton transport on InP, whereas the process is kinetically limited on GaP. This allows for spatial separation of individual stages of hydrogen-evolving, multistep reactions on InP(001). Possible implications for the mechanisms of cathodic water splitting and photocorrosion on the two surfaces are considered in light of available experimental evidence. C1 [Wood, Brandon C.; Schwegler, Eric; Choi, Woon Ih; Ogitsu, Tadashi] Lawrence Livermore Natl Lab, Quantum Simulat Grp, Livermore, CA 94550 USA. RP Wood, BC (reprint author), Lawrence Livermore Natl Lab, Quantum Simulat Grp, Livermore, CA 94550 USA. EM brandonwood@llnl.gov RI Schwegler, Eric/A-2436-2016; OI Schwegler, Eric/0000-0003-3635-7418; Choi, Woon Ih/0000-0002-7183-3400 FU U.S. Department of Energy Fuel Cell Technologies Program; U.S. Department of Energy by LLNL [DE-AC52-07NA27344] FX We acknowledge helpful discussions with J. Turner, T. Deutsch, and H. Wang (NREL), and with D. Esposito (NIST). Funding was provided by the U.S. Department of Energy Fuel Cell Technologies Program. Computing support came from the Lawrence Livermore National Laboratory (LLNL) Institutional Computing Grand Challenge program. This work was performed under the auspices of the U.S. Department of Energy by LLNL under Contract DE-AC52-07NA27344. NR 67 TC 18 Z9 18 U1 5 U2 104 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 EI 1520-5126 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD OCT 23 PY 2013 VL 135 IS 42 BP 15774 EP 15783 DI 10.1021/ja403850s PG 10 WC Chemistry, Multidisciplinary SC Chemistry GA 242CV UT WOS:000326215900025 PM 24053479 ER PT J AU Snyder, RA Bell, CB Diao, YH Krebs, C Bollinger, JM Solomon, EI AF Snyder, Rae Ana Bell, Caleb B., III Diao, Yinghui Krebs, Carsten Bollinger, J. Martin, Jr. Solomon, Edward I. TI Circular Dichroism, Magnetic Circular Dichroism, and Variable Temperature Variable Field Magnetic Circular Dichroism Studies of Biferrous and Mixed-Valent myo-Inositol Oxygenase: Insights into Substrate Activation of O-2 Reactivity SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID METHANE MONOOXYGENASE HYDROXYLASE; COLI RIBONUCLEOTIDE REDUCTASE; METHYLOCOCCUS-CAPSULATUS BATH; IRON ACTIVE-SITE; GLUCURONIC-ACID; PEROXODIFERRIC INTERMEDIATE; ELECTRONIC-STRUCTURE; CRYSTAL-STRUCTURE; RADICAL COFACTOR; INOSITOL AB myo-Inositol oxygenase (MIOX) catalyzes the 4(e)(-) oxidation of myo-inositol (MI) to D-glucuronate using a substrate activated Fe(II)Fe(III) site. The biferrous and Fe(II)Fe(III) forms of MIOX were studied with circular dichroism (CD), magnetic circular dichroism (MCD), and variable temperature variable field (VTVH) MCD spectroscopies. The MCD spectrum of biferrous MIOX shows two ligand field (LF) transitions near 10000 cm(-1), split by similar to 2000 cm(-1), characteristic of six coordinate (6C) Fe(II) sites, indicating that the modest reactivity of the biferrous form toward O-2 can be attributed to the saturated coordination of both irons. Upon oxidation to the Fe(II)Fe(III) state, MIOX shows two LF transitions in the similar to 10000 cm(-1) region, again implying a coordinatively saturated Fe(II) site. Upon MI binding, these split in energy to 5200 and 11200 cm(-1), showing that MI binding causes the Fe(II) to become coordinatively unsaturated. VTVH MCD magnetization curves of unbound and MI-bound Fe(II)Fe(III) forms show that upon substrate binding, the isotherms become more nested, requiring that the exchange coupling and ferrous zero-field splitting (ZFS) both decrease in magnitude. These results imply that MI binds to the ferric site, weakening the Fe(III)-mu-OH bond and strengthening the Fe(II)-mu-OH bond. This perturbation results in the release of a coordinated water from the Fe(II) that enables its O-2 activation. C1 [Snyder, Rae Ana; Bell, Caleb B., III; Solomon, Edward I.] Stanford Univ, Dept Chem, Stanford, CA 94305 USA. [Diao, Yinghui; Krebs, Carsten; Bollinger, J. Martin, Jr.] Penn State Univ, Dept Biochem & Mol Biol, University Pk, PA 16802 USA. [Krebs, Carsten; Bollinger, J. Martin, Jr.] Penn State Univ, Dept Chem, University Pk, PA 16802 USA. [Solomon, Edward I.] Stanford Univ, SLAC, Stanford Synchrotron Radiat Lab, Menlo Pk, CA 94025 USA. RP Krebs, C (reprint author), Penn State Univ, Dept Biochem & Mol Biol, University Pk, PA 16802 USA. EM ckrebs@psu.edu; jmb21@psu.edu; edward.solomon@stanford.edu RI Krebs, Carsten/D-4773-2009; Bollinger, Joseph /C-1425-2016 OI Krebs, Carsten/0000-0002-3302-7053; FU NSF Biochemistry Program Grant [MCB-0919027]; National Institutes of Health [DK-074641] FX The NSF Biochemistry Program Grant (MCB-0919027 to E.I.S.) and the National Institutes of Health (Grant DK-074641 to J.M.B. and C.K.) provided financial support for this research. NR 71 TC 2 Z9 2 U1 3 U2 26 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 EI 1520-5126 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD OCT 23 PY 2013 VL 135 IS 42 BP 15851 EP 15863 DI 10.1021/ja406635k PG 13 WC Chemistry, Multidisciplinary SC Chemistry GA 242CV UT WOS:000326215900033 PM 24066857 ER PT J AU Feng, XW Mathoniere, C Jeon, IR Rouzieres, M Ozarowski, A Aubrey, ML Gonzalez, MI Clerac, R Long, JR AF Feng, Xiaowen Mathoniere, Corine Jeon, Ie-Rang Rouzieres, Mathieu Ozarowski, Andrew Aubrey, Michael L. Gonzalez, Miguel I. Clerac, Rodolphe Long, Jeffrey R. TI Tristability in a Light-Actuated Single-Molecule Magnet SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID SPIN-CROSSOVER SYSTEMS; IRON(II) COMPLEXES; RELAXATION; STATE; TRANSITION; SUSCEPTIBILITY; FE(PTZ)6(BF4)2; CRYSTAL; LIGANDS; MEMORY AB Molecules exhibiting bistability have been proposed as elementary binary units (bits) for information storage, potentially enabling fast and efficient computing. In particular, transition metal complexes can display magnetic bistability via either spin-crossover or single-molecule magnet behavior. We now show that the octahedral iron(II) complexes in the molecular salt [Fe(1-propyltetrazole)(6)](BF4)(2), when placed in its high-symmetry form, can combine both types of behavior. Light irradiation under an applied magnetic field enables fully reversible switching between an S = 0 state and an S = 2 state with either up (M-S = +2) or down (M-S = -2) polarities. The resulting tristability suggests the possibility of using molecules for ternary information storage in direct analogy to current binary systems that employ magnetic switching and the magneto-optical Kerr effect as write and read mechanisms. C1 [Feng, Xiaowen; Aubrey, Michael L.; Gonzalez, Miguel I.; Long, Jeffrey R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Mathoniere, Corine; Jeon, Ie-Rang] CNRS, ICMCB, UPR 9048, F-33600 Pessac, France. [Mathoniere, Corine; Jeon, Ie-Rang] Univ Bordeaux, ICMCB, UPR 9048, F-33600 Pessac, France. [Jeon, Ie-Rang; Rouzieres, Mathieu; Clerac, Rodolphe] CNRS, CRPP, UPR 8641, Res Team Mol Magnet Mat, F-33600 Pessac, France. [Jeon, Ie-Rang; Rouzieres, Mathieu; Clerac, Rodolphe] Univ Bordeaux, CRPP, UPR 8641, F-33600 Pessac, France. [Ozarowski, Andrew] Natl High Magnet Field Lab, Tallahassee, FL 32310 USA. [Long, Jeffrey R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Clerac, R (reprint author), CNRS, CRPP, UPR 8641, Res Team Mol Magnet Mat, F-33600 Pessac, France. EM clerac@crpp-bordeaux.cnrs.fr; jrlong@berkeley.edu OI Gonzalez, Miguel/0000-0003-4250-9035; Jeon, Ie-Rang/0000-0001-5509-169X FU National Science Foundation [CHE-1010002]; Centre National de la Recherche Scientifique (CNRS); University of Bordeaux; Conseil Regional d'Aquitaine; GIS Advanced Materials in Aquitaine (COMET Project); ANR [NT09_469563]; Institut Universitaire de France (IUF); NSF Grant [DMR-1157490]; State of Florida FX Research carried out at the University of California, Berkeley was supported by National Science Foundation Grant CHE-1010002. Research in France was funded by the Centre National de la Recherche Scientifique (CNRS), the University of Bordeaux, the Conseil Regional d'Aquitaine, GIS Advanced Materials in Aquitaine (COMET Project), the ANR (NT09_469563, AC-MAGnets Project), and Institut Universitaire de France (IUF). A portion of the work was performed at the National High Magnetic Field Laboratory and was supported by NSF Grant DMR-1157490 and the State of Florida. We thank Dr. T. D. Harris for helpful discussions. NR 35 TC 47 Z9 47 U1 3 U2 75 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD OCT 23 PY 2013 VL 135 IS 42 BP 15880 EP 15884 DI 10.1021/ja407332y PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA 242CV UT WOS:000326215900036 PM 24066720 ER PT J AU Malliakas, CD Poineau, F Johnstone, EV Weck, PF Kim, E Scott, BL Forster, PM Kanatzidis, MG Czerwinski, KR Sattelberger, AP AF Malliakas, Christos D. Poineau, Frederic Johnstone, Erik V. Weck, Philippe F. Kim, Eunja Scott, Brian L. Forster, Paul M. Kanatzidis, Mercouri G. Czerwinski, Kenneth R. Sattelberger, Alfred P. TI beta-Technetium Dichloride: Solid-State Modulated Structure, Electronic Structure, and Physical Properties SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID GENERALIZED GRADIENT APPROXIMATION; CRENEL FUNCTIONS; CHLORIDE; CLUSTERS; HALIDES; PLATINUM; METALS; MOLYBDENUM; ZIRCONIUM; PT6CL12 AB A second polymorph of technetium dichloride, beta-TcCl2, has been synthesized from the reaction of Tc metal and chlorine in a sealed tube at 450 degrees C. The crystallographic structure and physical properties of beta-TcCl2 have been investigated. The structure of beta-TcCl2 consists of infinite chains of face sharing [Tc2Cl8] units; within a chain, the Tc Tc vectors of two adjacent [Tc2Cl8] units are ordered in the long-range where perpendicular and/or parallel arrangement of Tc Tc vectors yields a modulated structure. Resistivity and Seebeck measurements performed on a beta-TcCl2 single crystal indicate the compound to be a p-type semiconductor while a magnetic susceptibility measurement shows technetium dichloride to be diamagnetic. A band gap of 0.12(2) eV was determined by reflectance spectroscopy measurements. Theoretical calculations at the density functional level were utilized for the investigation of other possible stable forms of TcCl2. C1 [Malliakas, Christos D.; Kanatzidis, Mercouri G.; Sattelberger, Alfred P.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Poineau, Frederic; Johnstone, Erik V.; Forster, Paul M.; Czerwinski, Kenneth R.; Sattelberger, Alfred P.] Univ Nevada, Dept Chem, Las Vegas, NV 89154 USA. [Weck, Philippe F.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Kim, Eunja] Univ Nevada, Dept Phys & Astron, Las Vegas, NV 89154 USA. [Scott, Brian L.] Los Alamos Natl Lab, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA. [Malliakas, Christos D.; Kanatzidis, Mercouri G.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Sattelberger, Alfred P.] Argonne Natl Lab, Energy Engn & Syst Anal Directorate, Argonne, IL 60439 USA. RP Sattelberger, AP (reprint author), Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. EM asattelberger@anl.gov RI Scott, Brian/D-8995-2017; OI Scott, Brian/0000-0003-0468-5396; , Philippe/0000-0002-7610-2893 FU NEUP grant from the U.S. Department of Energy, Office of Nuclear Energy, through INL/BEA, LLC [00129169, DE-AC07-05ID14517]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX Funding for this research was provided by an NEUP grant from the U.S. Department of Energy, Office of Nuclear Energy, through INL/BEA, LLC, 00129169, agreement No. DE-AC07-05ID14517. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. The authors thank Trevor Low and Julie Bertoia for outstanding health physics support. This work was also supported by the U.S. Department of Energy, Office of Basic Energy Sciences under contract no. DE-AC02-06CH11357. NR 67 TC 3 Z9 3 U1 2 U2 18 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD OCT 23 PY 2013 VL 135 IS 42 BP 15955 EP 15962 DI 10.1021/ja408459k PG 8 WC Chemistry, Multidisciplinary SC Chemistry GA 242CV UT WOS:000326215900045 PM 24053573 ER PT J AU Bousso, R AF Bousso, Raphael TI Firewalls from double purity SO PHYSICAL REVIEW D LA English DT Article ID BLACK-HOLE EVAPORATION; THERMODYNAMICS; ENTROPY; PARTICLE; LAW AB The firewall paradox is often presented as arising from double entanglement, but I argue that more generally the paradox is double purity. Near-horizon modes are purified by the interior, in the infalling vacuum. Hence, they cannot also be pure alone, or in combination with any third system, as demanded by unitarity. This conflict arises independently of the Page time, for entangled and for pure states. It implies that identifications of Hilbert spaces cannot resolve the paradox. Traditional complementarity requires the unitary identification of infalling matter with a scrambled subsystem of the Hawking radiation. Extending this map to the infalling vacuum overdetermines the out-state. More general complementarity maps ("A = R-B," "ER = EPR") necessarily fail when the near-horizon zone is pure. I argue that pure-zone states span the microcanonical ensemble, and that this suffices to make the horizon a special place. I advocate that the ability to detect the horizon locally, rather than the degree or probability of violence, is what makes firewalls problematic. Conversely, if the production of matter at the horizon can be dynamically understood and shown to be consistent, then firewalls do not constitute a violation of the equivalence principle. C1 [Bousso, Raphael] Univ Calif Berkeley, Ctr Theoret Phys, Berkeley, CA 94720 USA. [Bousso, Raphael] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Bousso, Raphael] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Bousso, R (reprint author), Univ Calif Berkeley, Ctr Theoret Phys, Berkeley, CA 94720 USA. RI Bousso, Regina/F-5178-2012 OI Bousso, Regina/0000-0002-9250-0250 FU Berkeley Center for Theoretical Physics; National Science Foundation [1214644]; fqxi Grant [RFP3-1004]; U.S. Department of Energy [DE-AC02-05CH11231] FX I would like to thank the organizers of the CERN workshop on Black Hole Horizons and Quantum Information, March 2013, where the main results of this paper were first presented. (Video is available at http://cds.cern.ch/record/1532382.) I have benefitted from valuable discussions with many colleagues, especially S. Giddings, D. Harlow, D. Mainemer Katz, D. Marolf, J. Polchinski, V. Rosenhaus, D. Stanford, and L. Susskind. This work was supported by the Berkeley Center for Theoretical Physics, by the National Science Foundation (Grant No. 1214644), by fqxi Grant No. RFP3-1004, by "New Frontiers in Astronomy and Cosmology," and by the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 53 TC 27 Z9 27 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD OCT 23 PY 2013 VL 88 IS 8 AR 084035 DI 10.1103/PhysRevD.88.084035 PG 14 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 240PR UT WOS:000326109900004 ER PT J AU Iyer, S Karig, DK Norred, SE Simpson, ML Doktycz, MJ AF Iyer, Sukanya Karig, David K. Norred, S. Elizabeth Simpson, Michael L. Doktycz, Mitchel J. TI Multi-Input Regulation and Logic with T7 Promoters in Cells and Cell-Free Systems SO PLOS ONE LA English DT Article ID RNA-POLYMERASE MUTANTS; SYNTHETIC BIOLOGY; ESCHERICHIA-COLI; GENE REPRESSION; LAC REPRESSOR; IN-VIVO; TRANSCRIPTION; EXPRESSION; GATES; OPERATORS AB Engineered gene circuits offer an opportunity to harness biological systems for biotechnological and biomedical applications. However, reliance on native host promoters for the construction of circuit elements, such as logic gates, can make the implementation of predictable, independently functioning circuits difficult. In contrast, T7 promoters offer a simple orthogonal expression system for use in a variety of cellular backgrounds and even in cell-free systems. Here we develop a T7 promoter system that can be regulated by two different transcriptional repressors for the construction of a logic gate that functions in cells and in cell-free systems. We first present LacI repressible T7lacO promoters that are regulated from a distal lac operator site for repression. We next explore the positioning of a tet operator site within the T7lacO framework to create T7 promoters that respond to tet and lac repressors and realize an IMPLIES gate. Finally, we demonstrate that these dual input sensitive promoters function in an E. coli cell-free protein expression system. Our results expand the utility of T7 promoters in cell based as well as cell-free synthetic biology applications. C1 [Iyer, Sukanya; Doktycz, Mitchel J.] Univ Tennessee, Grad Program Genome Sci & Technol, Knoxville, TN USA. [Iyer, Sukanya; Doktycz, Mitchel J.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN USA. [Karig, David K.; Simpson, Michael L.; Doktycz, Mitchel J.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN USA. [Norred, S. Elizabeth; Simpson, Michael L.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Simpson, Michael L.] Univ Tennessee, Ctr Environm Biotechnol, Knoxville, TN 37932 USA. RP Doktycz, MJ (reprint author), Univ Tennessee, Grad Program Genome Sci & Technol, Knoxville, TN USA. EM doktyczmj@ornl.gov RI Simpson, Michael/A-8410-2011; Karig, David/G-5703-2011; Doktycz, Mitchel/A-7499-2011 OI Simpson, Michael/0000-0002-3933-3457; Karig, David/0000-0002-9508-6411; Doktycz, Mitchel/0000-0003-4856-8343 FU NIH [EB000657]; Center for Nanophase Materials Sciences; Oak Ridge National Laboratory by the Division of Scientific User Facilities, U.S. Department of Energy; U.S. DOE [DE-AC05- 00OR22725] FX work was supported by NIH Grant EB000657 and by the in-house research program of the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Division of Scientific User Facilities, U.S. Department of Energy. This work was performed at the Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. DOE under Contract No. DE-AC05- 00OR22725. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 64 TC 5 Z9 5 U1 2 U2 28 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD OCT 23 PY 2013 VL 8 IS 10 AR e78442 DI 10.1371/journal.pone.0078442 PG 12 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 239PE UT WOS:000326037000112 PM 24194933 ER PT J AU Sato, R Shirai, S Tobioka, K AF Sato, Ryosuke Shirai, Satoshi Tobioka, Kohsaku TI Flavor of gluino decay in high-scale supersymmetry SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Supersymmetry Phenomenology ID SPLIT SUPERSYMMETRY; STANDARD MODEL; DARK-MATTER; BOSON MASS; RADIATIVE-CORRECTIONS; ANOMALY MEDIATION; WINO LSP; LHC; BREAKING; SEARCHES AB The discovery of the Higgs boson with a mass of about 125 GeV intimates us a possibility of a high-scale supersymmetry (SUSY) breaking model, where a sfermion mass scale is much higher than the electroweak scale. Although a general SUSY standard model can contribute to the low-energy flavor and/or CP-violating processes, the high-scale SUSY breaking model provides smaller signatures and therefore are less constrained, even in the presence of large flavor/CP violations of sfermions. However, a manner of gluino decay directly reflects the squark flavor structure and provides us a clue for the sfermion flavor structure. In this paper, we study the gluino decay in detail and discuss the interplay with the gluino decay and low-energy flavor and CP observation. C1 [Sato, Ryosuke] High Energy Accelerator Res Org KEK, Inst Particle & Nucl Studies, Tsukuba, Ibaraki 3050801, Japan. [Shirai, Satoshi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Phys, Berkeley Ctr Theoret Phys, Berkeley, CA 94720 USA. [Shirai, Satoshi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Theoret Phys Grp, Berkeley, CA 94720 USA. [Tobioka, Kohsaku] Univ Tokyo, Dept Phys, Tokyo 1130033, Japan. [Tobioka, Kohsaku] Univ Tokyo, Todai Inst Adv Study, Kavli Inst Phys & Math Universe WPI, Kashiwa, Chiba 2778583, Japan. RP Sato, R (reprint author), High Energy Accelerator Res Org KEK, Inst Particle & Nucl Studies, Tsukuba, Ibaraki 3050801, Japan. EM rsato@post.kek.jp; shirai@berkeley.edu; kohsaku.tobioka@ipmu.jp OI Sato, Ryosuke/0000-0003-2745-4208 FU JSPS; World Premier International Research Center Initiative (WPI Initiative), MEXT, Japan FX SS thanks L. Hall and Y. Nomura for fruitful discussion. The work of RS and KT is supported in part by JSPS Research Fellowships for Young Scientists. This work is also supported by the World Premier International Research Center Initiative (WPI Initiative), MEXT, Japan. NR 71 TC 11 Z9 11 U1 0 U2 3 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD OCT 23 PY 2013 IS 10 AR 157 DI 10.1007/JHEP10(2013)157 PG 26 WC Physics, Particles & Fields SC Physics GA 239TE UT WOS:000326047600003 ER PT J AU Kormann, F Grabowski, B Soderlind, P Palumbo, M Fries, SG Hickel, T Neugebauer, J AF Koermann, F. Grabowski, B. Soederlind, P. Palumbo, M. Fries, S. G. Hickel, T. Neugebauer, J. TI Thermodynamic modeling of chromium: strong and weak magnetic coupling SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article ID SPIN-DENSITY-WAVE; THERMAL-EXPANSION; LOW-TEMPERATURES; HEAT-CAPACITIES; ALLOYS; CR; ANTIFERROMAGNETISM; FLUCTUATIONS; EXCITATIONS; TRANSITION AB As chromium is a decisive ingredient for stainless steels, a reliable understanding of its thermodynamic properties is indispensable. Parameter-free first-principles methods have nowadays evolved to a state allowing such thermodynamic predictions. For materials such as Cr, however, the inclusion of magnetic entropy and higher order contributions such as anharmonic entropy is still a formidable task. Employing state-of-the-art ab initio molecular dynamics simulations and statistical concepts, we compute a set of thermodynamic properties based on quasiharmonic, anharmonic, electronic and magnetic free energy contributions from first principles. The magnetic contribution is modeled by an effective nearest-neighbor Heisenberg model, which itself is solved numerically exactly by means of a quantum Monte Carlo method. We investigate two different scenarios: a weak magnetic coupling scenario for Cr, as usually presumed in empirical thermodynamic models, turns out to be in clear disagreement with experimental observations. We show that instead a mixed Hamiltonian including weak and strong magnetic coupling provides a consistent picture with good agreement to experimental thermodynamic data. C1 [Koermann, F.; Grabowski, B.; Hickel, T.; Neugebauer, J.] Max Planck Inst Eisenforsch GmbH, D-40237 Dusseldorf, Germany. [Soederlind, P.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Palumbo, M.; Fries, S. G.] Ruhr Univ Bochum, ICAMS, D-44780 Bochum, Germany. RP Kormann, F (reprint author), Max Planck Inst Eisenforsch GmbH, D-40237 Dusseldorf, Germany. EM koermann@mpie.de RI Kormann, Fritz/A-5677-2012; Grabowski, Blazej/D-8430-2012; Neugebauer, Joerg/K-2041-2015 OI Kormann, Fritz/0000-0003-3050-6291; Grabowski, Blazej/0000-0003-4281-5665; Neugebauer, Joerg/0000-0002-7903-2472 FU Deutsche Forschungsgemeinschaft [SFB 761]; Interdisciplinary Centre for Advanced Materials Simulation (ICAMS); ThyssenKrupp AG; Bayer MaterialScience AG; Salzgitter Mannesmann Forschung GmbH; Robert Bosch GmbH; Benteler Stahl/Rohr GmbH; Bayer Technology Services GmbH; state of North-Rhine Westphalia; European Commission; European Research Council [290998]; US Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX Funding by the collaborative research center SFB 761 'Stahl-ab initio' of the Deutsche Forschungsgemeinschaft and the Interdisciplinary Centre for Advanced Materials Simulation (ICAMS), which is supported by ThyssenKrupp AG, Bayer MaterialScience AG, Salzgitter Mannesmann Forschung GmbH, Robert Bosch GmbH, Benteler Stahl/Rohr GmbH, Bayer Technology Services GmbH and the state of North-Rhine Westphalia as well as the European Commission in the framework of the European Regional Development Fund (ERDF), is gratefully acknowledged. The funding by the European Research Council under the EU's 7th Framework Programme (FP7/2007-2013)/ERC Grant agreement 290998 is gratefully acknowledged. Part of this work was performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 64 TC 9 Z9 9 U1 2 U2 28 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD OCT 23 PY 2013 VL 25 IS 42 AR 425401 DI 10.1088/0953-8984/25/42/425401 PG 7 WC Physics, Condensed Matter SC Physics GA 230KK UT WOS:000325337700006 PM 24065339 ER PT J AU McLerran, L Praszalowicz, M Schenke, B AF McLerran, Larry Praszalowicz, Michal Schenke, Bjoern TI Transverse momentum of protons, pions and kaons in high multiplicity pp and pA collisions: Evidence for the color glass condensate? SO NUCLEAR PHYSICS A LA English DT Article DE High-energy nuclear collisions; Color glass condensate ID GLUON DISTRIBUTION-FUNCTIONS; LARGE NUCLEI; 7 TEV; HADRON; QCD; LHC AB The CMS experiment at the Large Hadron Collider has recently presented data on the average transverse momentum of protons, kaons and pions as a function of particle multiplicity. We relate the particle multiplicity to saturation momentum using recently published computations of the interaction radius determined from the theory of the Color Glass Condensate. We show that the pp and the pA experimental data scale in terms of these saturation momenta. Computing transverse momentum spectra for identified particles using Boltzmann-type distributions and relating different associated multiplicities using geometric scaling, these simple distributions reproduce the observed dependence of the mean transverse momentum on particle multiplicities seen in both pp and pA interactions for pions to good accuracy, and to fair agreement for protons and kaons. (C) 2013 Elsevier B.V. All rights reserved. C1 [McLerran, Larry; Schenke, Bjoern] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [McLerran, Larry] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. [McLerran, Larry] Cent China Normal Univ, Dept Phys, Wuhan 430079, Peoples R China. [Praszalowicz, Michal] Jagellonian Univ, M Smoluchowski Inst Phys, PL-30059 Krakow, Poland. RP Schenke, B (reprint author), Brookhaven Natl Lab, Dept Phys, Bldg 510A, Upton, NY 11973 USA. EM bschenke@quark.phy.bnl.gov RI Praszalowicz, Michal/F-1912-2016 FU DOE [DEACO2-98CH10886.]; Polish NCN [2011/01/B/ST2100492] FX The research of L. McLerran and B. Schenke is supported under DOE Contract No. DEACO2-98CH10886. The research of M. Praszalowicz is supported by the Polish NCN grant 2011/01/B/ST2100492. NR 27 TC 26 Z9 26 U1 0 U2 4 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0375-9474 EI 1873-1554 J9 NUCL PHYS A JI Nucl. Phys. A PD OCT 23 PY 2013 VL 916 BP 210 EP 218 DI 10.1016/j.nuclphysa.2013.08.008 PG 9 WC Physics, Nuclear SC Physics GA 237WZ UT WOS:000325903500010 ER PT J AU Koehler, PE Larsen, AC Guttormsen, M Siem, S Guber, KH AF Koehler, P. E. Larsen, A. C. Guttormsen, M. Siem, S. Guber, K. H. TI Extreme nonstatistical effects in gamma decay of Mo-95 neutron resonances SO PHYSICAL REVIEW C LA English DT Article AB We demonstrate that high-quality total radiation width (Gamma(gamma)) data are a virtually untapped resource for testing and improving nuclear models. To this end, we obtained unprecedentedly large sets of Gamma(gamma) values for all six s- and p-wave J(pi) values for Mo-95 neutron resonances. We show that Gamma(gamma) distributions simulated in the framework of the nuclear statistical model are in sharp disagreement with the data. Simulations modified to include doorway effects resulted in much better agreement. These results call into question the reliability of the nuclear statistical model. C1 [Koehler, P. E.; Larsen, A. C.; Guttormsen, M.; Siem, S.] Univ Oslo, Dept Phys, N-0316 Oslo, Norway. [Guber, K. H.] Oak Ridge Natl Lab, Reactor & Nucl Syst Div, Oak Ridge, TN 37831 USA. RP Koehler, PE (reprint author), Univ Oslo, Dept Phys, N-0316 Oslo, Norway. RI Larsen, Ann-Cecilie/C-8742-2014; OI Larsen, Ann-Cecilie/0000-0002-2188-3709; Koehler, Paul/0000-0002-6717-0771 FU Research Council of Norway; Nuclear Criticality Safety Program; Office of Nuclear Physics of the US Department of Energy FX This work was supported by the Research Council of Norway and by the Nuclear Criticality Safety Program and the Office of Nuclear Physics of the US Department of Energy. NR 20 TC 6 Z9 6 U1 0 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD OCT 23 PY 2013 VL 88 IS 4 AR 041305 DI 10.1103/PhysRevC.88.041305 PG 5 WC Physics, Nuclear SC Physics GA 240LC UT WOS:000326096400001 ER PT J AU Danopoulos, S Parsa, S Al Alam, D Tabatabai, R Baptista, S Tiozzo, C Carraro, G Wheeler, M Barreto, G Braun, T Li, XK Hajihosseini, MK Bellusci, S AF Danopoulos, Soula Parsa, Sara Al Alam, Denise Tabatabai, Reza Baptista, Sheryl Tiozzo, Caterina Carraro, Gianni Wheeler, Matthew Barreto, Guillermo Braun, Thomas Li, Xiaokun Hajihosseini, Mohammad K. Bellusci, Saverio TI Transient Inhibition of FGFR2b-Ligands Signaling Leads to Irreversible Loss of Cellular beta-Catenin Organization and Signaling in AER during Mouse Limb Development SO PLOS ONE LA English DT Article ID APICAL ECTODERMAL RIDGE; MAMMARY-GLAND; DIFFERENTIATION; ORGANOGENESIS; MAINTENANCE; EXPRESSION; MISEXPRESSION; MORPHOGENESIS; COMPARTMENTS; INDUCTION AB The vertebrate limbs develop through coordinated series of inductive, growth and patterning events. Fibroblast Growth Factor receptor 2b (FGFR2b) signaling controls the induction of the Apical Ectodermal Ridge (AER) but its putative roles in limb outgrowth and patterning, as well as in AER morphology and cell behavior have remained unclear. We have investigated these roles through graded and reversible expression of soluble dominant-negative FGFR2b molecules at various times during mouse limb development, using a doxycycline/transactivator/tet(O)-responsive system. Transient attenuation (<= 24 hours) of FGFR2b-ligands signaling at E8.5, prior to limb bud induction, leads mostly to the loss or truncation of proximal skeletal elements with less severe impact on distal elements. Attenuation from E9.5 onwards, however, has an irreversible effect on the stability of the AER, resulting in a progressive loss of distal limb skeletal elements. The primary consequences of FGFR2b-ligands attenuation is a transient loss of cell adhesion and down-regulation of P63, beta 1-integrin and E-cadherin, and a permanent loss of cellular beta-catenin organization and WNT signaling within the AER. Combined, these effects lead to the progressive transformation of the AER cells from pluristratified to squamous epithelial-like cells within 24 hours of doxycycline administration. These findings show that FGFR2b-ligands signaling has critical stage-specific roles in maintaining the AER during limb development. C1 [Danopoulos, Soula; Parsa, Sara; Baptista, Sheryl; Bellusci, Saverio] Univ So Calif, Keck Sch Med, Los Angeles, CA 90033 USA. [Danopoulos, Soula; Parsa, Sara; Al Alam, Denise; Tabatabai, Reza; Tiozzo, Caterina; Bellusci, Saverio] Childrens Hosp Los Angeles, Saban Res Inst, Dev Biol & Regenerat Med Program, Los Angeles, CA 90027 USA. [Parsa, Sara] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. [Tiozzo, Caterina] Nassau Univ, Med Ctr, Dept Pediat, New York, NY USA. [Carraro, Gianni; Bellusci, Saverio] Univ Giessen, Lung Ctr, Dept Internal Med 2, D-35390 Giessen, Germany. [Wheeler, Matthew; Braun, Thomas] Max Planck Inst Heart & Lung Res, Dept Cardiac Dev & Remodelling, Bad Nauheim, Germany. [Barreto, Guillermo] Max Planck Inst Heart & Lung Res, LOEWE Res Grp Lung Canc Epigenet, Bad Nauheim, Germany. [Li, Xiaokun] Wenzhou Med Coll, Sch Pharm, Wenzhou, Peoples R China. [Hajihosseini, Mohammad K.] Univ E Anglia, Sch Biol Sci, Norwich NR4 7TJ, Norfolk, England. RP Bellusci, S (reprint author), Univ So Calif, Keck Sch Med, Los Angeles, CA 90033 USA. EM sbellusci@chla.usc.edu RI Braun, Thomas/B-2310-2008 FU American Lung Association; NIH [HL086322, HD052609, HL074832]; DFG, LOEWE initiative; Excellence Cluster in Cardio-Pulmonary system, Giessen, Germany FX D.A.A. acknowledges the support of the American Lung Association. S. B. acknowledges support from NIH (HL086322, HD052609 and HL074832) and DFG, LOEWE initiative as well as the Excellence Cluster in Cardio-Pulmonary system, Giessen, Germany. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 33 TC 7 Z9 7 U1 0 U2 4 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD OCT 22 PY 2013 VL 8 IS 10 AR e76248 DI 10.1371/journal.pone.0076248 PG 16 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 239OF UT WOS:000326034500003 PM 24167544 ER PT J AU Odokonyero, D Ragumani, S Lopez, MS Bonanno, JB Ozerova, NDS Woodard, DR Machala, BW Swaminathan, S Burley, SK Almo, SC Glasner, ME AF Odokonyero, Denis Ragumani, Sugadev Lopez, Mariana S. Bonanno, Jeffrey B. Ozerova, Nicole D. S. Woodard, DaNae R. Machala, Benjamin W. Swaminathan, Subramanyam Burley, Stephen K. Almo, Steven C. Glasner, Margaret E. TI Divergent Evolution of Ligand Binding in the o-Succinylbenzoate Synthase Family SO BIOCHEMISTRY LA English DT Article ID ACYLAMINO ACID RACEMASE; ENOLASE SUPERFAMILY; ENZYMATIC-ACTIVITIES; MANDELATE RACEMASE; ESCHERICHIA-COLI; ACTIVE-SITE; CRYSTAL-STRUCTURE; DEHYDRATASE; MECHANISM; RESIDUES AB Thermobifida fusca o-succinylbenzoate synthase (OSBS), a member of the enolase superfamily that catalyzes a step in menaquinone biosynthesis, has an amino acid sequence that is 22 and 28% identical with those of two previously characterized OSBS enzymes from Escherichia coli and Amycolatopsis sp. T-1-60, respectively. These values are considerably lower than typical levels of sequence identity among homologous proteins that have the same function. To determine how such divergent enzymes catalyze the same reaction, we determined the structure of T. fusca OSBS and identified amino acids that are important for ligand binding, significant differences in structure and conformational flexibility between T. fusca OSBS and other members of the enolase superfamily. In particular, the 20s loop, a flexible loop in the active site that permits ligand binding and release in most enolase superfamily proteins, has a four-amino acid deletion and is well-ordered in T. fusca OSBS. Instead, the flexibility of a different region allows the substrate to enter from the other side of the active site. T. fusca OSBS was more tolerant of mutations at residues that were critical for activity in E. coli OSBS. Also, replacing active site amino acids found in one protein with the amino acids that occur at the same place in the other protein reduces the catalytic efficiency. Thus, the extraordinary divergence between these proteins does not appear to reflect a higher tolerance of mutations. Instead, large deletions outside the active site were accompanied by alteration of active site size and electrostatic interactions, resulting in small but significant differences in ligand binding. C1 [Odokonyero, Denis; Lopez, Mariana S.; Ozerova, Nicole D. S.; Woodard, DaNae R.; Machala, Benjamin W.; Glasner, Margaret E.] Texas A&M Univ, Dept Biochem & Biophys, College Stn, TX 77843 USA. [Ragumani, Sugadev; Swaminathan, Subramanyam] Brookhaven Natl Lab, Dept Biosci, Upton, NY 11973 USA. [Burley, Stephen K.] Rutgers State Univ, Rutgers Canc Inst New Jersey, Ctr Integrat Prote Res, Res Collaboratory Struct Bioinformat Prot Data Ba, Piscataway, NJ 08854 USA. [Burley, Stephen K.] Rutgers State Univ, Dept Chem & Chem Biol, Piscataway, NJ 08854 USA. [Bonanno, Jeffrey B.; Almo, Steven C.] Albert Einstein Coll Med, Dept Biochem, Bronx, NY 10461 USA. [Almo, Steven C.] Albert Einstein Coll Med, Dept Physiol & Biophys, Bronx, NY 10461 USA. RP Glasner, ME (reprint author), Texas A&M Univ, Dept Biochem & Biophys, College Stn, TX 77843 USA. EM margy.glasner@tamu.edu OI Glasner, Margaret/0000-0003-1818-1965 FU Robert A. Welch Foundation [A-1758]; National Institutes of Health (NIH) [U54 GM074945, U54 GM094662]; National Institute of Biomedical Imaging and Bioengineering [P30-EB-009998]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX This work was supported by Grant A-1758 from the Robert A. Welch Foundation (Principle Investigator, M.E.G.). The NYSGXRC was supported by National Institutes of Health (NIH) Grant U54 GM074945 (Principal Investigator, S.K.B.). The NYSGRC is supported by NIH Grant U54 GM094662 (Principal Investigator, S.C.A.). The Center for Synchrotron Biosciences, where diffraction data were collected, was supported by Grant P30-EB-009998 from the National Institute of Biomedical Imaging and Bioengineering. Use of the National Synchrotron Light Source, Brookhaven National Laboratory, was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract DE-AC02-98CH10886. NR 45 TC 10 Z9 10 U1 1 U2 5 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0006-2960 J9 BIOCHEMISTRY-US JI Biochemistry PD OCT 22 PY 2013 VL 52 IS 42 BP 7512 EP 7521 DI 10.1021/bi401176d PG 10 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA 242AH UT WOS:000326209300016 PM 24060347 ER PT J AU Liu, J Yu, XQ Hu, EY Nam, KW Yang, XQ Khalifah, PG AF Liu, Jue Yu, Xiqian Hu, Enyuan Nam, Kyung-Wan Yang, Xiao-Qing Khalifah, Peter G. TI Divalent Iron Nitridophosphates: A New Class of Cathode Materials for Li-Ion Batteries SO CHEMISTRY OF MATERIALS LA English DT Article DE Na2Fe2P3O9N; Li2Fe2P3O9N; CUBICON; ion-exchange; Li-ion battery; cathode; cyclic voltammetry ID FLUOROPHOSPHATE C1 [Liu, Jue; Khalifah, Peter G.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Yu, Xiqian; Hu, Enyuan; Nam, Kyung-Wan; Yang, Xiao-Qing; Khalifah, Peter G.] Brookhaven Natl Lab, Dept Chem, New York, NY 11973 USA. RP Yang, XQ (reprint author), Brookhaven Natl Lab, Dept Chem, New York, NY 11973 USA. EM xyang@bnl.gov; kpete@bnl.gov RI Nam, Kyung-Wan/B-9029-2013; LIU, JUE/J-6463-2014; Hu, Enyuan/D-7492-2016; Yu, Xiqian/B-5574-2014; LIU, JUE/I-8631-2016 OI Nam, Kyung-Wan/0000-0001-6278-6369; LIU, JUE/0000-0003-1834-0356; Hu, Enyuan/0000-0002-1881-4534; Yu, Xiqian/0000-0001-8513-518X; LIU, JUE/0000-0002-4453-910X FU Northeastern Center for Chemical Energy Storage (NECCES); Energy Frontier Research Center; U.S. Department of Energy, Office of Basic Energy Sciences [DE-SC0001294, DE-AC02-98CH10886]; NYSTAR-NYSDED; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX Research was supported as part of the Northeastern Center for Chemical Energy Storage (NECCES), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Basic Energy Sciences, under Award DE-SC0001294, including matching support from NYSTAR-NYSDED. This research utilized the facilities at the Center for Functional Nanomaterials and the National Synchrotron Light Source, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. Research conducted at ORNL's Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. The authors thank Dr. Jianming Bai for beamline X14A assistance, Dr. Yuri Janssen for discussions on and implementation of BVS maps, Dr. Mikhail Feygeson and Dr. Jorg Neuefeind for NOMAD beamline assistance, and Ms. Bingfei Cao for neutron data collection. NR 11 TC 6 Z9 6 U1 4 U2 48 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD OCT 22 PY 2013 VL 25 IS 20 BP 3929 EP 3931 DI 10.1021/cm402567e PG 3 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA 242AG UT WOS:000326209200001 ER PT J AU George, NC Pell, AJ Dantelle, G Page, K Llobet, A Balasubramanian, M Pintacuda, G Chmelka, BF Seshadri, R AF George, Nathan C. Pell, Andrew J. Dantelle, Geraldine Page, Katharine Llobet, Anna Balasubramanian, M. Pintacuda, Guido Chmelka, Bradley F. Seshadri, Ram TI Local Environments of Dilute Activator Ions in the Solid-State Lighting Phosphor Y3-xCexAl5O12 SO CHEMISTRY OF MATERIALS LA English DT Article DE inorganic phosphors; white solid-state lighting structure-property relations; electron and nuclear magnetic resonance; X-ray and neutron scattering X-ray absorption ID YTTRIUM-ALUMINUM-GARNET; SPIN-LATTICE-RELAXATION; NUCLEAR-MAGNETIC-RESONANCE; PARAMAGNETIC SHIFT PROBES; BOND-VALENCE PARAMETERS; EMITTING-DIODES; MAS-NMR; LUMINESCENT PROPERTIES; OPTICAL-ABSORPTION; CRYSTAL-STRUCTURE AB The oxide garnet Y3Al5O12 (YAG), when substituted with a few percent of the activator ion Ce3+ to replace Y3+, is a luminescent material that is nearly ideal for phosphor-converted solid-state white lighting. The local environments of the small number of substituted Ce3+ ions are known to critically influence the optical properties of the phosphor. Using a combination of powerful experimental methods, the nature of these local environments is determined and is correlated with the macroscopic luminescent properties of Ce-substituted YAG. The rigidity of the garnet structure is established and is shown to play a key role in the high quantum yield and in the resistance toward thermal quenching of luminescence. Local structural probes reveal compression of the Ce3+ local environments by the rigid YAG structure, which gives rise to the unusually large crystal-field splitting, and hence yellow emission. Effective design rules for finding new phosphor materials inferred from the results establish that efficient phosphors require rigid, highly three-dimensionally connected host structures with simple compositions that manifest a low number of phonon modes, and low activator ion concentrations to avoid quenching. C1 [George, Nathan C.; Chmelka, Bradley F.] Univ Calif Santa Barbara, Dept Chem Engn, Santa Barbara, CA 93106 USA. [Pell, Andrew J.; Pintacuda, Guido] Univ Lyon 1, Ecole Normale Super Lyon, CNRS, Ctr RMN Tres Hauts Champs,UMR 5280, F-69100 Villeurbanne, France. [Dantelle, Geraldine] Ecole Polytech, Lab Phys Matiere Condensee, UMR 7643, CNRS, F-91128 Palaiseau, France. [Page, Katharine; Llobet, Anna] Los Alamos Natl Lab, Lujan Neutron Scattering Ctr, Los Alamos, NM 87545 USA. [Balasubramanian, M.] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. [Seshadri, Ram] Univ Calif Santa Barbara, Mat Dept, Santa Barbara, CA 93106 USA. [Seshadri, Ram] Univ Calif Santa Barbara, Mat Res Lab, Santa Barbara, CA 93106 USA. [George, Nathan C.; Seshadri, Ram] Univ Calif Santa Barbara, Mitsubishi Chem Ctr Adv Mat, Santa Barbara, CA 93106 USA. RP Chmelka, BF (reprint author), Univ Calif Santa Barbara, Dept Chem Engn, Santa Barbara, CA 93106 USA. EM bradc@engineering.ucsb.edu; seshadri@mrl.ucsb.edu RI Seshadri, Ram/C-4205-2013; Page, Katharine/C-9726-2009; Llobet, Anna/B-1672-2010; Dantelle, Geraldine/C-8296-2017 OI Seshadri, Ram/0000-0001-5858-4027; Page, Katharine/0000-0002-9071-3383; Dantelle, Geraldine/0000-0001-5499-8070 FU ConvEne IGERT Program of the U.S. NSF [NSF-DGE 0801627]; LABEX iMUST of the Universite de Lyon [ANR-10-LABX-0064, ANR-11-IDEX-0007]; MRSEC Program of the NSF [DMR-1121053]; Center for Scientific Computing at UCSB; NSF MRSEC [DMR-1121053]; NSF [CNS-0960316]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; DOE Office of Basic Energy Sciences; LANL [DE-AC52-06NA25396]; Agence Nationale de la Recherche [ANR 08-BLAN-0035-01] FX The authors thank Dr. R. Davis for advice on EXAFS fitting, Dr. A. Mikhailovsky for assistance with the quantum efficiency measurements, J. Siewenie for assistance with collection of the neutron powder diffraction data, Dr. Z. Gan for assistance with the 89Y NMR measurements, and Prof. C. Oertel for helpful suggestions on the manuscript. N.C.G. has been supported by the ConvEne IGERT Program of the U.S. NSF (NSF-DGE 0801627). A.J.P. and G.P. were supported by the LABEX iMUST (ANR-10-LABX-0064) of the Universite de Lyon, within the program "Investissements d'Avenir" (ANR-11-IDEX-0007) operated by the Agence Nationale de la Recherche (ANR). The research made extensive use of the Central Facilities of the UCSB Materials Research Laboratory, supported by the MRSEC Program of the NSF under Award DMR-1121053, which is a member of the NSF-funded Materials Research Facilities Network (www.mrfn.org). We acknowledge support from the Center for Scientific Computing at UCSB, supported by NSF MRSEC (DMR-1121053) and NSF CNS-0960316. Use of the Advanced Photon Source at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under contract no. DE-AC02-06CH11357. This work benefited from the use of NPDF and HIPD at the Lujan Center at Los Alamos National Laboratory, funded by DOE Office of Basic Energy Sciences; LANL is operated by Los Alamos National Security LLC under DE-AC52-06NA25396. The solid-state NMR measurements at 23.5 T were conducted at the Centre Europeen Champs Haute RMN in Lyon, France. A.J.P. and G.P. are supported by the Agence Nationale de la Recherche (ANR 08-BLAN-0035-01). Solid-state NMR measurements were conducted at the U.S. National High Magnetic Field Laboratory, Tallahassee, Florida, supported by the U.S. National Science Foundation. B.F.C. thanks the ENS-Lyon for support as a "Professeur Invite" in 2012. NR 126 TC 49 Z9 49 U1 6 U2 97 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD OCT 22 PY 2013 VL 25 IS 20 BP 3979 EP 3995 DI 10.1021/cm401598n PG 17 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA 242AG UT WOS:000326209200007 ER PT J AU Mohanty, D Huq, A Payzant, EA Sefat, AS Li, JL Abraham, DP Wood, DL Daniel, C AF Mohanty, Debasish Huq, Ashfia Payzant, E. Andrew Sefat, Athena S. Li, Jianlin Abraham, Daniel P. Wood, David L., III Daniel, Claus TI Neutron Diffraction and Magnetic Susceptibility Studies on a High-Voltage Li1.2Mn0.55Ni0.15Co0.10O2 Lithium Ion Battery Cathode: Insight into the Crystal Structure SO CHEMISTRY OF MATERIALS LA English DT Article DE lithium; and manganese-rich cathode; lithium ion batteries; neutron diffraction; magnetic ordering ID X-RAY-DIFFRACTION; LOCAL-STRUCTURE; ELECTRON-MICROSCOPY; SOLID-SOLUTION; TRANSFORMATION; MANGANESE; PERFORMANCE; HYSTERESIS; LI2MNO3; HOLD AB Lithium- and manganese-rich oxides undergo structural transformation and/or atomic rearrangements during the delithiation/lithiation process and ultimately suffer from several issues such as first cycle irreversible capacity and voltage fade. In order to understand the mechanism of these issues, perception of a detailed crystal structure of pristine material is obviously demanding. In this study, combined powder neutron diffraction (ND) and temperature-dependent magnetic susceptibility techniques were employed to investigate the structure of a pristine lithium- and manganese-rich Li1.2Mn0.55Ni0.15Co0.10O2 cathode oxide. Rietveld refinement on the experimental ND pattern yields good fits by considering either Li2MO3 (M = Co, Mn, Ni) type monoclinic (C2/m space group) phase with 1% of Ni residing in the 4h lithium site or a composite structure consisting of 50% of Li2MnO3 type monoclinic (C2/m space group) and 50% LiMO2 (M = Co, Mn, Ni) type trigonal (R (3) over barm space group) structure. In the composite structure, 3% Li/Ni site exchange in the trigonal phase is also proposed. Further, temperature-dependent dc magnetic susceptibility shows Curie-Weiss paramagnetic behavior at T >= 100 K, and no ordering/deviation of the field cooling (FC) curve in the temperature range 2-320 K indicates the random distribution of metal ions in the transition metal (TM) layer in the trigonal phase. Bifurcation of the zero-field cooling (ZFC) curve from the FC curve showing a magnetic ordering at T-N similar to SO K reveals the presence of cation ordering in the TM layers arising from a distinct Li2MnO3-like phase. These results suggest that the lithium- and manganese-rich oxide with a composition Li1.2Mn0.55Ni0.15Co0.10O2 is more likely a composite of monoclinic and trigonal phases. The report also highlights the unique materials diagnostic capability of combined ND and magnetic susceptibility techniques to obtain detailed structural information of complex oxide systems. C1 [Mohanty, Debasish; Sefat, Athena S.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37931 USA. [Huq, Ashfia; Payzant, E. Andrew] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37931 USA. [Li, Jianlin; Wood, David L., III; Daniel, Claus] Oak Ridge Natl Lab, Energy & Transportat Sci Div, Oak Ridge, TN 37931 USA. [Abraham, Daniel P.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Wood, David L., III; Daniel, Claus] Univ Tennessee, Bredesen Ctr Interdisciplinary Res & Grad Educ, Knoxville, TN 37996 USA. RP Mohanty, D (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37931 USA. EM mohantyd@ornl.gov; danielc@ornl.gov RI Payzant, Edward/B-5449-2009; Huq, Ashfia/J-8772-2013; Daniel, Claus/A-2060-2008; Mohanty, Debasish/B-6207-2012; Li, Jianlin/D-3476-2011; Sefat, Athena/R-5457-2016 OI Payzant, Edward/0000-0002-3447-2060; Wood, David/0000-0002-2471-4214; Huq, Ashfia/0000-0002-8445-9649; Daniel, Claus/0000-0002-0571-6054; Mohanty, Debasish/0000-0003-1141-0657; Li, Jianlin/0000-0002-8710-9847; Sefat, Athena/0000-0002-5596-3504 FU U.S. Department of Energy (DOE) [DE-AC05-00OR22725]; Vehicle Technologies Office Applied Battery Research Program (Program Managers Peter Faguy and David Howell) of the Office of Energy Efficiency and Renewable Energy; DOE Office of Basic Energy Sciences, Materials Sciences and Engineering Division; ORNL; Scientific User Facilities Division, Office of Basic Energy Sciences FX This research at Oak Ridge National Laboratory, managed by UT Battelle, LLC, for the U.S. Department of Energy (DOE) under contract DE-AC05-00OR22725, was sponsored by the Vehicle Technologies Office Applied Battery Research Program (Program Managers Peter Faguy and David Howell) of the Office of Energy Efficiency and Renewable Energy. This research was supported by the DOE Office of Basic Energy Sciences, Materials Sciences and Engineering Division and by ORNL's User Facility at the Spallation Neutron Source, which is sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences. The TODA HE5050 material was obtained from Argonne National Laboratory in collaboration with Andrew Jansen and Bryant Polzin. The authors thank Dr. Jason R. Croy from Argonne National Laboratory for his valuable suggestions on structural analysis. NR 35 TC 30 Z9 30 U1 8 U2 132 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD OCT 22 PY 2013 VL 25 IS 20 BP 4064 EP 4070 DI 10.1021/cm402278q PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA 242AG UT WOS:000326209200016 ER PT J AU Retuerto, M Emge, T Hadermann, J Stephens, PW Li, MR Yin, ZP Croft, M Ignatov, A Zhang, SJ Yuan, Z Jin, C Simonson, JW Aronson, MC Pan, A Basov, DN Kotliar, G Greenblatt, M AF Retuerto, M. Emge, T. Hadermann, J. Stephens, P. W. Li, M. R. Yin, Z. P. Croft, M. Ignatov, A. Zhang, S. J. Yuan, Z. Jin, C. Simonson, J. W. Aronson, M. C. Pan, A. Basov, D. N. Kotliar, G. Greenblatt, M. TI Synthesis and Properties of Charge-Ordered Thallium Halide Perovskites, CsTl0.5+Tl0.53+X3 (X = F or Cl): Theoretical Precursors for Superconductivity? SO CHEMISTRY OF MATERIALS LA English DT Article DE superconductivity; mixed valence; charge order; CsTlCl3; CsTlF3; CsAuCl3; BaBiO3 ID CRYSTAL-STRUCTURE; RAY-ABSORPTION; PHASE-DIAGRAM; SYSTEM; BAPB1-XBIXO3; CS2AUAUCL6; OXYGEN; STATE; BR; CU AB Recently, CsTlCl3 and CsTlF3 perovskites were theoretically predicted to be potential superconductors if they were optimally doped. The syntheses of these two compounds together with a complete characterization of the samples are reported. CsTlCl3 was obtained as orange crystals in two different polymorphs: a tetragonal phase (I4/m) and a cubic phase (Fm (3) over barm). CsTlF3 was formed as a light brown powder, and also as a double cubic perovskite (Fm (3) over barm). In all three CsTlX3 phases, Tl+ and Tl3+ were located in two different crystallographic positions that accommodate their different bond lengths. In CsTlCl3, some Tl vacancies were found in the Tl+ position. The charge ordering between Tl+ and Tl3+ was confirmed by X-ray absorption and Raman spectroscopy. The Raman spectroscopy of CsTlCl3 at high pressure (58 GPa) did not indicate any phase transition to a possible single Tl2+ state. However, the highly insulating material became less resistive with an increasing high pressure, while it underwent a change in its optical properties, from transparent to deeply opaque red, indicative of a decrease in the magnitude of the band gap. The theoretical design and experimental validation of the existence of CsTlF3 and CsTlCl3 cubic perovskites are the necessary first steps in confirming the theoretical prediction of superconductivity in these materials. C1 [Retuerto, M.; Emge, T.; Li, M. R.; Greenblatt, M.] Rutgers State Univ, Dept Chem & Chem Biol, Piscataway, NJ 08854 USA. [Hadermann, J.] Univ Antwerp, Dept Phys, EMAT, B-2020 Antwerp, Belgium. [Stephens, P. W.; Simonson, J. W.; Aronson, M. C.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Yin, Z. P.; Croft, M.; Ignatov, A.; Kotliar, G.] Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08854 USA. [Zhang, S. J.; Yuan, Z.; Jin, C.] Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China. [Aronson, M. C.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Pan, A.; Basov, D. N.] Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. RP Greenblatt, M (reprint author), Rutgers State Univ, Dept Chem & Chem Biol, 610 Taylor Rd, Piscataway, NJ 08854 USA. EM martha@rutchem.rutgers.edu RI Li, Manrong/C-2632-2011; Retuerto, Maria/D-6425-2014; Li, Man-Rong/D-1697-2012; Hadermann, Joke/F-4644-2011 OI Retuerto, Maria/0000-0001-7564-3500; Li, Man-Rong/0000-0001-8424-9134; FU National Science Foundation [DMR-0966829]; U.S. Department of Defense [VV911NF-12-1-0172]; Rutgers University (BOG); AFOSR-MURI program; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX This work was supported by National Science Foundation Grant DMR-0966829, U.S. Department of Defense Grant VV911NF-12-1-0172, and Rutgers University (BOG) grants. Z.P.Y. and G.K. were supported by the AFOSR-MURI program for better and higher temperature superconductors. Use of the National Synchrotron Light Source, Brookhaven National Laboratory, was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract DE-AC02-98CH10886. We thank Dr. Hongbing Sun and James Elliott for their help with the ICP and IR measurements. NR 44 TC 6 Z9 6 U1 4 U2 37 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD OCT 22 PY 2013 VL 25 IS 20 BP 4071 EP 4079 DI 10.1021/cm402423x PG 9 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA 242AG UT WOS:000326209200017 ER PT J AU Chen, MS Niskala, JR Unruh, DA Chu, CK Lee, OP Frechet, JMJ AF Chen, Mark S. Niskala, Jeremy R. Unruh, David A. Chu, Crystal K. Lee, Olivia P. Frechet, Jean M. J. TI Control of Polymer-Packing Orientation in Thin Films through Synthetic Tailoring of Backbone Coplanarity SO CHEMISTRY OF MATERIALS LA English DT Article DE conjugated polymers; packing orientation; backbone coplanarity; isoindigo; organic field-effect transistors; organic photovoltaics ID FIELD-EFFECT TRANSISTORS; HETEROJUNCTION SOLAR-CELLS; SHORT-CIRCUIT CURRENT; CONJUGATED POLYMERS; CHARGE-TRANSPORT; ORGANIC SEMICONDUCTORS; SIDE-CHAINS; OPTOELECTRONIC DEVICES; MOLECULAR ORDER; LIQUID-CRYSTAL AB Controlling solid-state order of pi-conjugated polymers through macromolecular design is essential for achieving high electronic device performance; yet, it remains a challenge, especially with respect to polymer-packing orientation. Our work investigates the influence of backbone coplanarity on a polymer's preference to pack face-on or edge-on relative to the substrate. Isoindigo-based polymers were synthesized with increasing planarity by systematically substituting thiophenes for phenyl rings in the acceptor comonomer. This increasing backbone coplanarity, supported by density functional theory (DFT) calculations of representative trimers, leads to the narrowing of polymer band gaps as characterized by ultraviolet-visible-near infrared (UV-vis-NIR) spectroscopy and cyclic voltammetry. Among the polymers studied, regiosymmetric II and TII polymers exhibited the highest hole mobilities in organic field-effect transistors (OFETs), while in organic photovoltaics (OPVs), TBII polymers that display intermediate levels of planarity provided the highest power conversion efficiencies. Upon thin-film analysis by atomic force microscropy (AFM) and grazing-incidence X-ray diffraction (GIXD), we discovered that polymer-packing orientation could be controlled by tuning polymer planarity and solubility. Highly soluble, planar polymers favor face-on orientation in thin films while the less soluble, nonplanar polymers favor an edge-on orientation. This study advances our fundamental understanding of how polymer structure influences nanostructural order and reveals a new synthetic strategy for the design of semiconducting materials with rationally engineered solid-state properties. C1 [Chen, Mark S.; Niskala, Jeremy R.; Unruh, David A.; Chu, Crystal K.; Lee, Olivia P.; Frechet, Jean M. J.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Chen, Mark S.; Niskala, Jeremy R.; Unruh, David A.; Chu, Crystal K.; Lee, Olivia P.; Frechet, Jean M. J.] Univ Calif Berkeley, Dept Chem Engn, Berkeley, CA 94720 USA. [Chen, Mark S.; Niskala, Jeremy R.; Unruh, David A.; Lee, Olivia P.; Frechet, Jean M. J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Frechet, Jean M. J.] King Abdullah Univ Sci & Technol, Thuwal 239556900, Saudi Arabia. RP Chen, MS (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM mschen@berkeley.edu; jean.frechet@kaust.edu.sa OI Frechet, Jean /0000-0001-6419-0163 FU King Abdullah University of Science and Technology (KAUST) through the Center for Advanced Molecular Photovoltaics (CAMP) [KUS-C1-015-21]; Frechet "various gifts" fund; Camille and Henry Dreyfus Postdoctoral Program in Environmental Chemistry FX This work was supported in part by King Abdullah University of Science and Technology (KAUST) through the Center for Advanced Molecular Photovoltaics (CAMP) under Award No. KUS-C1-015-21, and the Frechet "various gifts" fund for the support of research in new materials. Portions of this research were carried out at the Stanford Synchrotron Radiation Lightsource user facility, operated on behalf of the U.S. Department of Energy, Office of Basic Energy Sciences. M.S.C. thanks the Camille and Henry Dreyfus Postdoctoral Program in Environmental Chemistry for a fellowship; the assistance of Jessica C. Moreton is acknowledged with thanks. NR 92 TC 97 Z9 97 U1 13 U2 121 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD OCT 22 PY 2013 VL 25 IS 20 BP 4088 EP 4096 DI 10.1021/cm402489a PG 9 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA 242AG UT WOS:000326209200019 ER PT J AU Deshmukh, P Ahn, SK de Merxem, LG Kasi, RM AF Deshmukh, Prashant Ahn, Suk-kyun de Merxem, Ludovic Geelhand Kasi, Rajeswari M. TI Interplay between Liquid Crystalline Order and Microphase Segregation on the Self-Assembly of Side-Chain Liquid Crystalline Brush Block Copolymers SO MACROMOLECULES LA English DT Article ID DIBLOCK COPOLYMERS; FUNCTIONAL MATERIALS; POLYMER BRUSHES; PHASE-BEHAVIOR; MESOGEN; MICROSTRUCTURE; MORPHOLOGY; KINETICS; SERIES; BULK AB Herein we investigate the influence of competing self-organizing phenomena on the hierarchical self-assembly of liquid crystalline brush block copolymers (LCBBCs). A library of LCBBCs are synthesized using ring-opening metathesis polymerization (ROMP) of norbornene side-chain functionalized monomers comprising (1) cholesteryl mesogen with nine methylene spacer and (2) semicrystalline poly(ethylene glycol) (PEG). The self assembly of LCBBCs with variations in LC block content (7-80 wt %) are investigated in their melt state. All LCBBCs show two distinct thermal transitions corresponding to PEG semicrystalline phase and LC mesophases. Interestingly, the LCBBCs display a multilevel hierarchical structure evidenced by the results from X-ray scattering and transmission electron microscopy (TEM): (1) smectic A (SmA) mesophases (d = 3-7 nm) by the assembly of cholesteryl side chains and (2) microphase segregation into lamellar or cylinder (d = 40-75 nm) resulting from the incompatibility between LC moieties and PEG side chain. Surprisingly, the presence of microphase-segregated domains in LCBBCs prevents the formation of cholesteric mesophase in sharp contrast to side-chain liquid crystalline homopolymer (SCLCP) bearing the same mesogen and the flexible spacer. This could be attributed to very high surface to volume ratio at intermaterial dividing surface (IMDS) in LCBBCs, by which only LC layers (i.e., SmA mesophase) are favored to form at the IMDS. On the fundamental side, these LCBBCs are an interesting scaffold to explore the impact of interactions between LC order and microphase segregation of side-chain polymeric brushes on the self-assembly of LCBBCs. Moreover, these new LCBBC scaffolds will serve as a tool box for rational design of hierarchically organized functional materials for stimuli responsive applications. C1 [Deshmukh, Prashant; Kasi, Rajeswari M.] Univ Connecticut, Dept Chem, Storrs, CT 06269 USA. [Ahn, Suk-kyun] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [de Merxem, Ludovic Geelhand] Univ Rouen, Dept Chem, F-76821 Rouen, Haute Normandie, France. [Ahn, Suk-kyun; Kasi, Rajeswari M.] Univ Connecticut, Inst Mat Sci, Polymer Program, Storrs, CT 06269 USA. RP Kasi, RM (reprint author), Univ Connecticut, Dept Chem, Storrs, CT 06269 USA. EM kasi@ims.uconn.edu RI deshmukh, prashant/E-6834-2012 OI deshmukh, prashant/0000-0001-6973-027X FU University of Connecticut Research Foundation Faculty Grant, NSF CAREER Award [DMR-0748398] FX Financial support was provided University of Connecticut Research Foundation Faculty Grant, NSF CAREER Award to R.M.K (DMR-0748398). Central instrumentation facilities in the Institute of Materials Science, Chemistry Department, and the TEM facility at Physiology and Neurobiology (PNB) are acknowledged. We also thank Stephen Daniels for sectioning samples and performing TEM experiments. The authors are very thankful to the NSF-MRSEC X-ray Scattering Laboratory at University of Massachusetts Amherst for using their Rigaku-Molmet SAXS equipment and Dr. Dhanasekaran Thirunavukkarasu for helpful assistance with SAXS data collection. We also thank Dr. Manesh Gopinadhan and Prof. Chinedum O. Osuji (Yale University) for helpful discussions. NR 58 TC 19 Z9 19 U1 5 U2 65 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD OCT 22 PY 2013 VL 46 IS 20 BP 8245 EP 8252 DI 10.1021/ma401448j PG 8 WC Polymer Science SC Polymer Science GA 242AI UT WOS:000326209400019 ER PT J AU Chilikin, K Mizuk, R Adachi, I Aihara, H Arinstein, K Asner, DM Aulchenko, V Aushev, T Aziz, T Bakich, AM Bala, A Bhardwaj, V Bhuyan, B Bondar, A Bonvicini, G Bozek, A Bracko, M Brodzicka, J Browder, TE Chekelian, V Chen, A Chen, P Cheon, BG Chistov, R Cho, IS Cho, K Chobanova, V Choi, SK Choi, Y Cinabro, D Dalseno, J Danilov, M Dolezal, Z Dutta, D Eidelman, S Epifanov, D Farhat, H Fast, JE Ferber, T Frey, A Gaur, V Gabyshev, N Ganguly, S Gillard, R Goh, YM Golob, B Haba, J Hara, T Hayasaka, K Hayashii, H Horii, Y Hoshi, Y Hou, WS Hyun, HJ Iijima, T Ishikawa, A Itoh, R Iwasaki, Y Julius, T Kah, DH Kang, JH Kato, E Kawasaki, T Kichimi, H Kiesling, C Kim, DY Kim, HJ Kim, JB Kim, JH Kim, KT Kim, YJ Kinoshita, K Klucar, J Ko, BR Kodys, P Korpar, S Krizan, P Krokovny, P Kumita, T Kuzmin, A Kwon, YJ Lange, JS Lee, SH Li, J Li, Y Libby, J Liu, C Liu, Y Liventsev, D Lukin, P MacNaughton, J Matvienko, D Miyabayashi, K Miyata, H Mohanty, GB Moll, A Mori, T Muramatsu, N Mussa, R Nakano, E Nakao, M Natkaniec, Z Nayak, M Nedelkovska, E Ng, C Nisar, NK Nishida, S Nitoh, O Ogawa, S Okuno, S Olsen, SL Oswald, C Pakhlov, P Pakhlova, G Park, CW Park, H Park, HK Pedlar, TK Pestotnik, R Petric, M Piilonen, LE Ritter, M Rohrken, M Rostomyan, A Sahoo, H Saito, T Sakai, K Sakai, Y Sandilya, S Santel, D Santelj, L Sanuki, T Savinov, V Schneider, O Schnell, G Schwanda, C Semmler, D Senyo, K Seon, O Sevior, ME Shapkin, M Shen, CP Shibata, TA Shiu, JG Sibidanov, A Simon, F Sohn, YS Sokolov, A Solovieva, E Staric, M Steder, M Sumihama, M Sumiyoshi, T Tamponi, U Tanida, K Tatishvili, G Teramoto, Y Trabelsi, K Uchida, M Uehara, S Unno, Y Uno, S Urquijo, P Usov, Y Vahsen, SE Van Hulse, C Vanhoefer, P Varner, G Varvell, KE Vinokurova, A Vorobyev, V Wagner, MN Wang, CH Wang, MZ Wang, P Wang, XL Watanabe, M Watanabe, Y Williams, KM Won, E Yabsley, BD Yamamoto, H Yamashita, Y Yashchenko, S Yook, Y Yusa, Y Zhang, ZP Zhilich, V Zhulanov, V Zupanc, A AF Chilikin, K. Mizuk, R. Adachi, I. Aihara, H. Arinstein, K. Asner, D. M. Aulchenko, V. Aushev, T. Aziz, T. Bakich, A. M. Bala, A. Bhardwaj, V. Bhuyan, B. Bondar, A. Bonvicini, G. Bozek, A. Bracko, M. Brodzicka, J. Browder, T. E. Chekelian, V. Chen, A. Chen, P. Cheon, B. G. Chistov, R. Cho, I. -S. Cho, K. Chobanova, V. Choi, S. -K. Choi, Y. Cinabro, D. Dalseno, J. Danilov, M. Dolezal, Z. Dutta, D. Eidelman, S. Epifanov, D. Farhat, H. Fast, J. E. Ferber, T. Frey, A. Gaur, V. Gabyshev, N. Ganguly, S. Gillard, R. Goh, Y. M. Golob, B. Haba, J. Hara, T. Hayasaka, K. Hayashii, H. Horii, Y. Hoshi, Y. Hou, W. -S. Hyun, H. J. Iijima, T. Ishikawa, A. Itoh, R. Iwasaki, Y. Julius, T. Kah, D. H. Kang, J. H. Kato, E. Kawasaki, T. Kichimi, H. Kiesling, C. Kim, D. Y. Kim, H. J. Kim, J. B. Kim, J. H. Kim, K. T. Kim, Y. J. Kinoshita, K. Klucar, J. Ko, B. R. Kodys, P. Korpar, S. Krizan, P. Krokovny, P. Kumita, T. Kuzmin, A. Kwon, Y. -J. Lange, J. S. Lee, S. -H. Li, J. Li, Y. Libby, J. Liu, C. Liu, Y. Liventsev, D. Lukin, P. MacNaughton, J. Matvienko, D. Miyabayashi, K. Miyata, H. Mohanty, G. B. Moll, A. Mori, T. Muramatsu, N. Mussa, R. Nakano, E. Nakao, M. Natkaniec, Z. Nayak, M. Nedelkovska, E. Ng, C. Nisar, N. K. Nishida, S. Nitoh, O. Ogawa, S. Okuno, S. Olsen, S. L. Oswald, C. Pakhlov, P. Pakhlova, G. Park, C. W. Park, H. Park, H. K. Pedlar, T. K. Pestotnik, R. Petric, M. Piilonen, L. E. Ritter, M. Roehrken, M. Rostomyan, A. Sahoo, H. Saito, T. Sakai, K. Sakai, Y. Sandilya, S. Santel, D. Santelj, L. Sanuki, T. Savinov, V. Schneider, O. Schnell, G. Schwanda, C. Semmler, D. Senyo, K. Seon, O. Sevior, M. E. Shapkin, M. Shen, C. P. Shibata, T. -A. Shiu, J. -G. Sibidanov, A. Simon, F. Sohn, Y. -S. Sokolov, A. Solovieva, E. Staric, M. Steder, M. Sumihama, M. Sumiyoshi, T. Tamponi, U. Tanida, K. Tatishvili, G. Teramoto, Y. Trabelsi, K. Uchida, M. Uehara, S. Unno, Y. Uno, S. Urquijo, P. Usov, Y. Vahsen, S. E. Van Hulse, C. Vanhoefer, P. Varner, G. Varvell, K. E. Vinokurova, A. Vorobyev, V. Wagner, M. N. Wang, C. H. Wang, M. -Z. Wang, P. Wang, X. L. Watanabe, M. Watanabe, Y. Williams, K. M. Won, E. Yabsley, B. D. Yamamoto, H. Yamashita, Y. Yashchenko, S. Yook, Y. Yusa, Y. Zhang, Z. P. Zhilich, V. Zhulanov, V. Zupanc, A. CA Belle Collaboration TI Experimental constraints on the spin and parity of the Z(4430)(+) SO PHYSICAL REVIEW D LA English DT Article ID DETECTOR AB We perform a full amplitude analysis of B-0 -> psi'K+ pi(-) decays, with psi' -> mu + mu- or e+e -, to constrain the spin and parity of the Z(4430)-. The JP = 1(+) hypothesis is favored over the 0(-), 1(-), 2(-) and 2(+) hypotheses at the levels of 3: 4 sigma, 3: 7 sigma, 4: 7 sigma and 5.1 sigma , respectively. The analysis is based on a 711 fb(-1) data sample that contains 772 x 10(6) B (B) over bar pairs collected at the Upsilon(4S) resonance by the Belle detector at the asymmetric-energy e(+)e(-) collider KEKB. C1 [Schnell, G.; Van Hulse, C.] Univ Basque Country, UPV EHU, Bilbao 48080, Spain. [Oswald, C.; Urquijo, P.] Univ Bonn, D-53115 Bonn, Germany. [Arinstein, K.; Aulchenko, V.; Bondar, A.; Eidelman, S.; Gabyshev, N.; Krokovny, P.; Kuzmin, A.; Lukin, P.; Matvienko, D.; Usov, Y.; Vinokurova, A.; Vorobyev, V.; Zhilich, V.; Zhulanov, V.] Budker Inst Nucl Phys, SB RAS, Novosibirsk 630090, Russia. [Arinstein, K.; Aulchenko, V.; Bondar, A.; Eidelman, S.; Gabyshev, N.; Krokovny, P.; Kuzmin, A.; Lukin, P.; Matvienko, D.; Usov, Y.; Vinokurova, A.; Vorobyev, V.; Zhilich, V.; Zhulanov, V.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Dolezal, Z.; Kodys, P.] Charles Univ Prague, Fac Math & Phys, Prague 12116, Czech Republic. [Kinoshita, K.; Liu, Y.; Santel, D.] Univ Cincinnati, Cincinnati, OH 45221 USA. [Ferber, T.; Rostomyan, A.; Steder, M.; Yashchenko, S.] DESY, D-22607 Hamburg, Germany. [Lange, J. S.; Semmler, D.; Wagner, M. N.] Univ Giessen, D-35392 Giessen, Germany. [Sumihama, M.] Gifu Univ, Gifu 5011193, Japan. [Frey, A.] Univ Gottingen, Inst Phys 2, D-37073 Gottingen, Germany. [Choi, S. -K.] Gyeongsang Natl Univ, Chinju 660701, South Korea. [Cheon, B. G.; Goh, Y. M.; Unno, Y.] Hanyang Univ, Seoul 133791, South Korea. [Browder, T. E.; Sahoo, H.; Vahsen, S. E.; Varner, G.] Univ Hawaii, Honolulu, HI 96822 USA. [Adachi, I.; Haba, J.; Hara, T.; Itoh, R.; Iwasaki, Y.; Kichimi, H.; Liventsev, D.; MacNaughton, J.; Nakao, M.; Nishida, S.; Sakai, K.; Sakai, Y.; Trabelsi, K.; Uehara, S.; Uno, S.] High Energy Accelerator Res Org KEK, Tsukuba, Ibaraki 3050801, Japan. [Schnell, G.] Ikerbasque, Bilbao 48011, Spain. [Bhuyan, B.; Dutta, D.] Indian Inst Technol Guwahati, Gauhati 781039, Assam, India. [Libby, J.; Nayak, M.] Indian Inst Technol, Madras 600036, Tamil Nadu, India. [Wang, P.] Chinese Acad Sci, Inst High Energy Phys, Beijing 100049, Peoples R China. [Schwanda, C.] Inst High Energy Phys, A-1050 Vienna, Austria. [Shapkin, M.; Sokolov, A.] Inst High Energy Phys, Protvino 142281, Russia. [Mussa, R.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Chilikin, K.; Mizuk, R.; Aushev, T.; Chistov, R.; Danilov, M.; Pakhlov, P.; Pakhlova, G.; Solovieva, E.] Inst Theoret & Expt Phys, Moscow 117218, Russia. [Bracko, M.; Golob, B.; Klucar, J.; Korpar, S.; Krizan, P.; Pestotnik, R.; Petric, M.; Santelj, L.; Staric, M.] J Stefan Inst, Ljubljana 1000, Slovenia. [Okuno, S.; Watanabe, Y.] Kanagawa Univ, Yokohama, Kanagawa 2218686, Japan. [Roehrken, M.; Zupanc, A.] Karlsruhe Inst Technol, Inst Expt Kernphys, D-76131 Karlsruhe, Germany. [Cho, K.; Kim, J. H.; Kim, Y. J.] Korea Inst Sci & Technol Informat, Taejon 305806, South Korea. [Kim, J. B.; Kim, K. T.; Ko, B. R.; Lee, S. -H.; Won, E.] Korea Univ, Seoul 136713, South Korea. [Hyun, H. J.; Kah, D. H.; Kim, H. J.; Park, H.; Park, H. K.] Kyungpook Natl Univ, Taegu 702701, South Korea. [Schneider, O.] Ecole Polytech Fed Lausanne, CH-1015 Lausanne, Switzerland. [Golob, B.; Krizan, P.] Univ Ljubljana, Fac Math & Phys, Ljubljana 1000, Slovenia. [Pedlar, T. K.] Luther Coll, Decorah, IA 52101 USA. [Bracko, M.; Korpar, S.] Univ Maribor, SLO-2000 Maribor, Slovenia. [Chekelian, V.; Chobanova, V.; Dalseno, J.; Kiesling, C.; Moll, A.; Nedelkovska, E.; Ritter, M.; Simon, F.; Vanhoefer, P.] Max Planck Inst Phys & Astrophys, D-80805 Munich, Germany. [Julius, T.; Sevior, M. E.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Mizuk, R.; Danilov, M.; Pakhlov, P.] Moscow Engn Phys Inst, Moscow 115409, Russia. [Iijima, T.; Mori, T.; Seon, O.; Shen, C. P.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648602, Japan. [Hayasaka, K.; Horii, Y.; Iijima, T.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648602, Japan. [Bhardwaj, V.; Hayashii, H.; Miyabayashi, K.] Nara Womens Univ, Nara 6308506, Japan. [Chen, A.] Natl Cent Univ, Chungli 32054, Taiwan. [Wang, C. H.] Natl United Univ, Miaoli 36003, Taiwan. [Chen, P.; Hou, W. -S.; Shiu, J. -G.; Wang, M. -Z.] Natl Taiwan Univ, Dept Phys, Taipei 10617, Taiwan. [Bozek, A.; Brodzicka, J.; Natkaniec, Z.] H Niewodniczanski Inst Nucl Phys, PL-31342 Krakow, Poland. [Yamashita, Y.] Nippon Dent Univ, Niigata 9518580, Japan. [Kawasaki, T.; Miyata, H.; Watanabe, M.; Yusa, Y.] Niigata Univ, Niigata 9502181, Japan. [Nakano, E.; Teramoto, Y.] Osaka City Univ, Osaka 5588585, Japan. [Asner, D. M.; Fast, J. E.; Tatishvili, G.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Bala, A.] Panjab Univ, Chandigarh 160014, India. [Savinov, V.] Univ Pittsburgh, Pittsburgh, PA 15260 USA. [Muramatsu, N.] Tohoku Univ, Res Ctr Elect Photon Sci, Sendai, Miyagi 9808578, Japan. [Liu, C.; Zhang, Z. P.] Univ Sci & Technol China, Hefei 230026, Peoples R China. [Li, J.; Olsen, S. L.; Tanida, K.] Seoul Natl Univ, Seoul 151742, South Korea. [Kim, D. Y.] Soongsil Univ, Seoul 156743, South Korea. [Choi, Y.; Park, C. W.] Sungkyunkwan Univ, Suwon 440746, South Korea. [Bakich, A. M.; Sibidanov, A.; Varvell, K. E.; Yabsley, B. D.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Aziz, T.; Gaur, V.; Mohanty, G. B.; Nisar, N. K.; Sandilya, S.] Tata Inst Fundamental Res, Bombay 400005, Maharashtra, India. [Dalseno, J.; Moll, A.; Simon, F.] Tech Univ Munich, Excellence Cluster Universe, D-85748 Garching, Germany. [Ogawa, S.] Toho Univ, Chiba 2748510, Japan. [Hoshi, Y.] Tohoku Gakuin Univ, Tagajo, Miyagi 9858537, Japan. [Ishikawa, A.; Kato, E.; Saito, T.; Sanuki, T.; Yamamoto, H.] Tohoku Univ, Sendai, Miyagi 9808578, Japan. [Aihara, H.; Epifanov, D.; Ng, C.] Univ Tokyo, Dept Phys, Tokyo 1130033, Japan. [Shibata, T. -A.; Uchida, M.] Tokyo Inst Technol, Tokyo 1528550, Japan. [Kumita, T.; Sumiyoshi, T.] Tokyo Metropolitan Univ, Tokyo 1920397, Japan. [Nitoh, O.] Tokyo Univ Agr & Technol, Koganei, Tokyo 1848588, Japan. [Tamponi, U.] Univ Turin, I-10124 Turin, Italy. [Li, Y.; Piilonen, L. E.; Wang, X. L.; Williams, K. M.] Virginia Polytech Inst & State Univ, CNP, Blacksburg, VA 24061 USA. [Bonvicini, G.; Cinabro, D.; Farhat, H.; Ganguly, S.; Gillard, R.] Wayne State Univ, Detroit, MI 48202 USA. [Senyo, K.] Yamagata Univ, Yamagata 9908560, Japan. [Cho, I. -S.; Kang, J. H.; Kwon, Y. -J.; Sohn, Y. -S.; Yook, Y.] Yonsei Univ, Seoul 120749, South Korea. RP Chilikin, K (reprint author), Univ Basque Country, UPV EHU, Bilbao 48080, Spain. RI Nitoh, Osamu/C-3522-2013; Aihara, Hiroaki/F-3854-2010; Ishikawa, Akimasa/G-6916-2012; Pakhlov, Pavel/K-2158-2013; Danilov, Mikhail/C-5380-2014; Mizuk, Roman/B-3751-2014; Krokovny, Pavel/G-4421-2016; Chilikin, Kirill/B-4402-2014; Chistov, Ruslan/B-4893-2014; Pakhlova, Galina/C-5378-2014; Solovieva, Elena/B-2449-2014; OI Aihara, Hiroaki/0000-0002-1907-5964; Pakhlov, Pavel/0000-0001-7426-4824; Danilov, Mikhail/0000-0001-9227-5164; Krokovny, Pavel/0000-0002-1236-4667; Chilikin, Kirill/0000-0001-7620-2053; Chistov, Ruslan/0000-0003-1439-8390; Pakhlova, Galina/0000-0001-7518-3022; Solovieva, Elena/0000-0002-5735-4059; Trabelsi, Karim/0000-0001-6567-3036; WANG, MIN-ZU/0000-0002-0979-8341; Mussa, Roberto/0000-0002-0294-9071 FU Ministry of Education, Culture, Sports, Science, and Technology (MEXT) of Japan; Japan Society for the Promotion of Science (JSPS); Tau-Lepton Physics Research Center of Nagoya University; Australian Research Council and the Australian Department of Industry, Innovation, Science and Research; Austrian Science Fund [22742-N16]; National Natural Science Foundation of China [10575109, 10775142, 10875115]; Ministry of Education, Youth and Sports of the Czech Republic [MSM0021620859]; Carl Zeiss Foundation; Deutsche Forschungsgemeinschaft; Department of Science and Technology of India; Istituto Nazionale di Fisica Nucleare of Italy; BK21 and WCU programs of the Ministry of Education, Science and Technology; National Research Foundation of Korea [2010-0021174, 2011-0029457, 2012-0008143, 2012R1A1A2008330]; BRL [KRF-2011-0020333]; GSDC of the Korea Institute of Science and Technology Information; Polish Ministry of Science and Higher Education; National Science Center; Ministry of Education and Science of the Russian Federation; Russian Federal Agency for Atomic Energy and Russian Foundation [12-02-00862-a]; Slovenian Research Agency; the Basque Foundation for Science (IKERBASQUE); Swiss National Science Foundation; National Science Council and theMinistry of Education of Taiwan; U.S. Department of Energy and the National Science Foundation; MEXT FX We thank the KEKB group for the excellent operation of the accelerator; the KEK cryogenics group for the efficient operation of the solenoid; and the KEK computer group, the National Institute of Informatics, and the PNNL/EMSL computing group for valuable computing and SINET4 network support. We acknowledge support from the Ministry of Education, Culture, Sports, Science, and Technology (MEXT) of Japan, the Japan Society for the Promotion of Science (JSPS), and the Tau-Lepton Physics Research Center of Nagoya University; the Australian Research Council and the Australian Department of Industry, Innovation, Science and Research; the Austrian Science Fund under Grant No. P 22742-N16; the National Natural Science Foundation of China under Contracts No. 10575109, No. 10775142, No. 10875115, and No. 10825524; the Ministry of Education, Youth and Sports of the Czech Republic under Contract No. MSM0021620859; the Carl Zeiss Foundation, the Deutsche Forschungsgemeinschaft and the VolkswagenStiftung; the Department of Science and Technology of India; the Istituto Nazionale di Fisica Nucleare of Italy; the BK21 and WCU programs of the Ministry of Education, Science and Technology, National Research Foundation of Korea Grants No. 2010-0021174, No. 2011-0029457, No. 2012-0008143, and No. 2012R1A1A2008330, the BRL program under NRF Grant No. KRF-2011-0020333, and GSDC of the Korea Institute of Science and Technology Information; the Polish Ministry of Science and Higher Education and the National Science Center; the Ministry of Education and Science of the Russian Federation, the Russian Federal Agency for Atomic Energy and Russian Foundation for Basic Research under Grant No. 12-02-00862-a; the Slovenian Research Agency; the Basque Foundation for Science (IKERBASQUE) and the UPV/EHU under Program No. UFI 11/55; the Swiss National Science Foundation; the National Science Council and theMinistry of Education of Taiwan; and the U.S. Department of Energy and the National Science Foundation. This work is supported by a Grant-in-Aid from MEXT for Science Research in a Priority Area ("New Development of Flavor Physics''), and from JSPS for Creative Scientific Research ("Evolution of Tau-lepton Physics''). NR 20 TC 70 Z9 72 U1 0 U2 35 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD OCT 22 PY 2013 VL 88 IS 7 AR UNSP 074026 DI 10.1103/PhysRevD.88.074026 PG 12 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 240ON UT WOS:000326106600005 ER PT J AU Chern, GW Morrison, MJ Nisoli, C AF Chern, Gia-Wei Morrison, Muir J. Nisoli, Cristiano TI Degeneracy and Criticality from Emergent Frustration in Artificial Spin Ice SO PHYSICAL REVIEW LETTERS LA English DT Article ID SYSTEMS; DISORDER; ENTROPY AB Although initially introduced to mimic the spin-ice pyrochlores, no artificial spin ice has yet exhibited the expected degenerate ice phase with critical correlations similar to the celebrated Coulomb phase in the pyrochlore lattice. Here we study a novel artificial spin ice based on a vertex-frustrated rather than pairwise frustrated geometry and show that it exhibits a quasicritical ice phase of extensive residual entropy and, significantly, algebraic correlations. Interesting in its own regard as a novel realization of frustration in a vertex system, our lattice opens new pathways to study defects in a critical manifold and to design degeneracy in artificial magnetic nanoarrays, a task so far elusive. C1 [Chern, Gia-Wei] LANL, Div Theoret, Los Alamos, NM 87545 USA. LANL, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. RP Chern, GW (reprint author), LANL, Div Theoret, Los Alamos, NM 87545 USA. OI Nisoli, Cristiano/0000-0003-0053-1023 FU National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory [DEAC52-06NA25396]; LANL Oppenheimer Fellowship FX We thank P. Mellado, A. Libal, C. Reichhardt, and R. Moessner for useful comments. This work was carried out under the auspices of the National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory under Contract No. DEAC52-06NA25396. G. W. C. acknowledges the support of the LANL Oppenheimer Fellowship. NR 38 TC 16 Z9 16 U1 1 U2 34 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 22 PY 2013 VL 111 IS 17 AR 177201 DI 10.1103/PhysRevLett.111.177201 PG 5 WC Physics, Multidisciplinary SC Physics GA 241ED UT WOS:000326148300017 PM 24206515 ER PT J AU Santer, BD Painter, JF Bonfils, C Mears, CA Solomon, S Wigley, TML Gleckler, PJ Schmidt, GA Doutriaux, C Gillett, NP Taylor, KE Thorne, PW Wentz, FJ AF Santer, Benjamin D. Painter, Jeffrey F. Bonfils, Celine Mears, Carl A. Solomon, Susan Wigley, Tom M. L. Gleckler, Peter J. Schmidt, Gavin A. Doutriaux, Charles Gillett, Nathan P. Taylor, Karl E. Thorne, Peter W. Wentz, Frank J. TI Human and natural influences on the changing thermal structure of the atmosphere SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE climate change detection; climate modeling ID STRATOSPHERIC TEMPERATURE TRENDS; CLIMATE-CHANGE; ATTRIBUTION; SIMULATIONS; OZONE AB Since the late 1970s, satellite-based instruments have monitored global changes in atmospheric temperature. These measurements reveal multidecadal tropospheric warming and stratospheric cooling, punctuated by short-term volcanic signals of reverse sign. Similar long-and short-term temperature signals occur in model simulations driven by human-caused changes in atmospheric composition and natural variations in volcanic aerosols. Most previous comparisons of modeled and observed atmospheric temperature changes have used results from individual models and individual observational records. In contrast, we rely on a large multimodel archive and multiple observational datasets. We show that a human-caused latitude/altitude pattern of atmospheric temperature change can be identified with high statistical confidence in satellite data. Results are robust to current uncertainties in models and observations. Virtually all previous research in this area has attempted to discriminate an anthropogenic signal from internal variability. Here, we present evidence that a human-caused signal can also be identified relative to the larger "total" natural variability arising from sources internal to the climate system, solar irradiance changes, and volcanic forcing. Consistent signal identification occurs because both internal and total natural variability (as simulated by state-of-the-art models) cannot produce sustained global-scale tropospheric warming and stratospheric cooling. Our results provide clear evidence for a discernible human influence on the thermal structure of the atmosphere. C1 [Santer, Benjamin D.; Painter, Jeffrey F.; Bonfils, Celine; Gleckler, Peter J.; Doutriaux, Charles; Taylor, Karl E.] Lawrence Livermore Natl Lab, Program Climate Model Diag & Intercomparison, Livermore, CA 94550 USA. [Mears, Carl A.; Wentz, Frank J.] Remote Sensing Syst, Santa Rosa, CA 95401 USA. [Solomon, Susan] MIT, Cambridge, MA 02139 USA. [Wigley, Tom M. L.] Natl Ctr Atmospher Res, Boulder, CO 80307 USA. [Wigley, Tom M. L.] Univ Adelaide, Sch Earth & Environm Sci, Adelaide, SA 5005, Australia. [Schmidt, Gavin A.] NASA, Goddard Inst Space Studies, New York, NY 10025 USA. [Gillett, Nathan P.] Environm Canada, Canadian Ctr Climate Modelling & Anal, Victoria, BC V8W 2Y2, Canada. [Thorne, Peter W.] Nansen Environm & Remote Sensing Ctr, N-5006 Bergen, Norway. RP Santer, BD (reprint author), Lawrence Livermore Natl Lab, Program Climate Model Diag & Intercomparison, Livermore, CA 94550 USA. EM santer1@llnl.gov RI Santer, Benjamin/F-9781-2011; Schmidt, Gavin/D-4427-2012; Taylor, Karl/F-7290-2011; Gleckler, Peter/H-4762-2012; Thorne, Peter/F-2225-2014 OI Schmidt, Gavin/0000-0002-2258-0486; Taylor, Karl/0000-0002-6491-2135; Gleckler, Peter/0000-0003-2816-6224; Thorne, Peter/0000-0003-0485-9798 FU DOE [DE-AC52-07NA27344]; DOE/Office of Biological and Environmental Research (OBER) Early Career Research Program Award [SCW1295]; DOE/OBER [DE-AC52-07NA27344] FX We acknowledge the World Climate Research Programme's Working Group on Coupled Modelling, which is responsible for CMIP, and we thank the climate modeling groups (listed in SI Appendix, Table S1) for producing and making available their model output. For CMIP, the Department of Energy (DOE) Program for Climate Model Diagnosis and Intercomparison (PCMDI) provides coordinating support and led development of software infrastructure in partnership with the Global Organization for Earth System Science Portals. Helpful comments and advice were provided by Jim Boyle (PCMDI), Kerry Emanuel (Massachusetts Institute of Technology), and Mike MacCracken. At Lawrence Livermore National Laboratory, work by B. D. S., J.F.P., P.J.G., and K. E. T. was performed under the auspices of the DOE under Contract DE-AC52-07NA27344; C. B. was supported by the DOE/Office of Biological and Environmental Research (OBER) Early Career Research Program Award SCW1295; and C. D. was funded under DOE/OBER Contract DE-AC52-07NA27344. NR 36 TC 18 Z9 19 U1 8 U2 61 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD OCT 22 PY 2013 VL 110 IS 43 BP 17235 EP 17240 DI 10.1073/pnas.1305332110 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 238JU UT WOS:000325943300027 PM 24043789 ER PT J AU Brennecka, GA Borg, LE Wadhwa, M AF Brennecka, Gregory A. Borg, Lars E. Wadhwa, Meenakshi TI Evidence for supernova injection into the solar nebula and the decoupling of r-process nucleosynthesis SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE isotopic anomalies; early Solar System; H-Event; nebular disk ID REFRACTORY INCLUSIONS; ISOTOPIC ANOMALIES; PROTOPLANETARY DISK; ALLENDE METEORITE; SYSTEM; SAMARIUM; HETEROGENEITY; NEODYMIUM; BARIUM; STARS AB The isotopic composition of our Solar System reflects the blending of materials derived from numerous past nucleosynthetic events, each characterized by a distinct isotopic signature. We show that the isotopic compositions of elements spanning a large mass range in the earliest formed solids in our Solar System, calcium-aluminum-rich inclusions (CAIs), are uniform, and yet distinct from the average Solar System composition. Relative to younger objects in the Solar System, CAIs contain positive r-process anomalies in isotopes A < 140 and negative r-process anomalies in isotopes A > 140. This fundamental difference in the isotopic character of CAIs around mass 140 necessitates (i) the existence of multiple sources for r-process nucleosynthesis and (ii) the injection of supernova material into a reservoir untapped by CAIs. A scenario of late supernova injection into the protoplanetary disk is consistent with formation of our Solar System in an active star-forming region of the galaxy. C1 [Brennecka, Gregory A.; Borg, Lars E.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Brennecka, Gregory A.; Wadhwa, Meenakshi] Arizona State Univ, Sch Earth & Space Explorat, Tempe, AZ 85287 USA. RP Brennecka, GA (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM brennecka2@llnl.gov FU US Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; National Aeronautics and Space Administration [NNH08ZDA001N, NNX07AF49G] FX The authors would like to thank D. Papanastassiou and one anonymous reviewer, whose contributions significantly improved the manuscript and the presentation of the data. This work was performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. The portion of the work performed at Lawrence Livermore National Laboratory and Arizona State University were supported by National Aeronautics and Space Administration Cosmochemistry Grants NNH08ZDA001N (to L. E. B.) and NNX07AF49G (to M.W.). NR 42 TC 20 Z9 21 U1 3 U2 28 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD OCT 22 PY 2013 VL 110 IS 43 BP 17241 EP 17246 DI 10.1073/pnas.1307759110 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 238JU UT WOS:000325943300028 PM 24101483 ER PT J AU Wu, JJ Lin, JF Wang, XC Liu, QQ Zhu, JL Xiao, YM Chow, P Jin, CQ AF Wu, J. J. Lin, Jung-Fu Wang, X. C. Liu, Q. Q. Zhu, J. L. Xiao, Y. M. Chow, P. Jin, Changqing TI Pressure-decoupled magnetic and structural transitions of the parent compound of iron-based 122 superconductors BaFe2As2 SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE ferropnictide-type superconductor; high-pressure effect; spin order ID NUCLEAR RESONANT SCATTERING; ARSENIDE SUPERCONDUCTOR; NA1-XFEAS; PHASE AB The recent discovery of iron ferropnictide superconductors has received intensive concern in connection with magnetically involved superconductors. Prominent features of ferropnictide superconductors are becoming apparent: the parent compounds exhibit an antiferromagnetic ordered spin density wave (SDW) state, the magnetic-phase transition is always accompanied by a crystal structural transition, and superconductivity can be induced by suppressing the SDW phase via either chemical doping or applied external pressure to the parent state. These features generated considerable interest in the interplay between magnetism and structure in chemically doped samples, showing crystal structure transitions always precede or coincide with magnetic transition. Pressure-tuned transition, on the other hand, would be more straightforward to superconducting mechanism studies because there are no disorder effects caused by chemical doping; however, remarkably little is known about the interplay in the parent compounds under controlled pressure due to the experimental challenge of in situ measuring both of magnetic and crystal structure evolution at high pressure and low temperatures. Here we show from combined synchrotron Mossbauer and X-ray diffraction at high pressures that the magnetic ordering surprisingly precedes the structural transition at high pressures in the parent compound BaFe2As2, in sharp contrast to the chemical-doping case. The results can be well understood in terms of the spin fluctuations in the emerging nematic phase before the long-range magnetic order that sheds light on understanding how the parent compound evolves from a SDW state to a superconducting phase, a key scientific inquiry of iron-based superconductors. C1 [Wu, J. J.; Wang, X. C.; Liu, Q. Q.; Zhu, J. L.; Jin, Changqing] Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China. [Wu, J. J.; Lin, Jung-Fu] Univ Texas Austin, Jackson Sch Geosci, Dept Geol Sci, Austin, TX 78712 USA. [Xiao, Y. M.; Chow, P.] Argonne Natl Lab, High Pressure Collaborat Access Team, Carnegie Inst Washington, Adv Photon Source, Argonne, IL 60439 USA. RP Lin, JF (reprint author), Univ Texas Austin, Jackson Sch Geosci, Dept Geol Sci, Austin, TX 78712 USA. EM afu@jsg.utexas.edu; jin@iphy.ac.cn RI Lin, Jung-Fu/B-4917-2011 FU National Nuclear Security Administration, Department of Energy [DE-NA0001974]; Basic Energy Sciences, Department of Energy (DOE-BES) [DE-FG02-99ER45775]; National Science Foundation; DOE-BES [DE-AC02-06CH11357]; Energy Frontier Research in Extreme Environments (EFree); Carnegie/DOE Alliance Center; Ministry of Science and Technology of China FX We thank C. Kenney-Benson, J. Liu, and C. Lu for their assistance; Z. Mao for helping with data analyses; and A. Wheat for editing the manuscript. We are also grateful to Wenge Yang, Yusheng Zhao, and Guoyin Shen for discussions. Portions of this work were performed at the High Pressure Collaborative Access Team (HPCAT Sector 16), Advanced Photon Source, Argonne National Laboratory. HPCAT operations are supported by the National Nuclear Security Administration, Department of Energy under Award DE-NA0001974 and by the Basic Energy Sciences, Department of Energy (DOE-BES) under Award DE-FG02-99ER45775, with partial instrumentation funding by the National Science Foundation. Advanced Photon Source, Argonne National Laboratory is supported by DOE-BES under Contract DE-AC02-06CH11357. Work at The University of Texas at Austin is supported by Energy Frontier Research in Extreme Environments (EFree) and the Carnegie/DOE Alliance Center. Work at the Chinese Academy of Sciences is supported by National Science Foundation and Ministry of Science and Technology of China through research projects. NR 38 TC 14 Z9 14 U1 3 U2 44 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD OCT 22 PY 2013 VL 110 IS 43 BP 17263 EP 17266 DI 10.1073/pnas.1310286110 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 238JU UT WOS:000325943300032 PM 24101468 ER PT J AU Wier, AD Mayekar, MK Heroux, A Arndt, KM VanDemark, AP AF Wier, Adam D. Mayekar, Manasi K. Heroux, Annie Arndt, Karen M. VanDemark, Andrew P. TI Structural basis for Spt5-mediated recruitment of the Paf1 complex to chromatin SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE histone modification; scaffold; DSIF; Cdk9; crystallography ID RNA-POLYMERASE-II; COTRANSCRIPTIONAL HISTONE MODIFICATION; CARBOXYL-TERMINAL DOMAIN; TRANSCRIPTION ELONGATION; SACCHAROMYCES-CEREVISIAE; SPT4-SPT5 COMPLEX; SPT5; RTF1; PHOSPHORYLATION; METHYLATION AB Polymerase associated factor 1 complex (Paf1C) broadly influences gene expression by regulating chromatin structure and the recruitment of RNA-processing factors during transcription elongation. The Plus3 domain of the Rtf1 subunit mediates Paf1C recruitment to genes by binding a repeating domain within the elongation factor Spt5 (suppressor of Ty). Here we provide a molecular description of this interaction by reporting the structure of human Rtf1 Plus3 in complex with a phosphorylated Spt5 repeat. We find that Spt5 binding is mediated by an extended surface containing phosphothreonine recognition and hydrophobic interfaces that interact with residues outside the Spt5 motif. Changes within these interfaces diminish binding of Spt5 in vitro and chromatin localization of Rtf1 in vivo. The structure reveals the basis for recognition of the repeat motif of Spt5, a key player in the recruitment of gene regulatory factors to RNA polymerase II. C1 [Wier, Adam D.; Mayekar, Manasi K.; Arndt, Karen M.; VanDemark, Andrew P.] Univ Pittsburgh, Dept Biol Sci, Pittsburgh, PA 15260 USA. [Heroux, Annie] Brookhaven Natl Lab, Dept Biol, Upton, NY 11973 USA. RP VanDemark, AP (reprint author), Univ Pittsburgh, Dept Biol Sci, Pittsburgh, PA 15260 USA. EM andyv@pitt.edu FU National Institutes of Health [R01 GM52593] FX The authors thank B. Van Houten, B. Tomson, C. MacGillivray, and A. Berman for technical assistance and advice. Funding support was provided by National Institutes of Health Grant R01 GM52593 (to K.M.A.). NR 51 TC 18 Z9 18 U1 1 U2 9 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD OCT 22 PY 2013 VL 110 IS 43 BP 17290 EP 17295 DI 10.1073/pnas.1314754110 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 238JU UT WOS:000325943300037 PM 24101474 ER PT J AU Hura, GL Tsai, CL Claridge, SA Mendillo, ML Smith, JM Williams, GJ Mastroianni, AJ Alivisatos, AP Putnam, CD Kolodner, RD Tainer, JA AF Hura, Greg L. Tsai, Chi-Lin Claridge, Shelley A. Mendillo, Marc L. Smith, Jessica M. Williams, Gareth J. Mastroianni, Alexander J. Alivisatos, A. Paul Putnam, Christopher D. Kolodner, Richard D. Tainer, John A. TI DNA conformations in mismatch repair probed in solution by X-ray scattering from gold nanocrystals SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article ID ESCHERICHIA-COLI MUTS; SACCHAROMYCES-CEREVISIAE MSH2-MSH6; TETRAMERIZATION DOMAIN; PROTEIN MUTS; IN-VIVO; RECOGNITION; COMPLEX; DISTANCE; REVEALS; SAXS AB DNA metabolism and processing frequently require transient or metastable DNA conformations that are biologically important but challenging to characterize. We use gold nanocrystal labels combined with small angle X-ray scattering to develop, test, and apply a method to follow DNA conformations acting in the Escherichia coli mismatch repair (MMR) system in solution. We developed a neutral PEG linker that allowed gold-labeled DNAs to be flash-cooled and stored without degradation in sample quality. The 1,000-fold increased gold nanocrystal scattering vs. DNA enabled investigations at much lower concentrations than otherwise possible to avoid concentration-dependent tetramerization of the MMR initiation enzyme MutS. We analyzed the correlation scattering functions for the nanocrystals to provide higher resolution inter-particle distributions not convoluted by the intraparticle distribution. We determined that mispair-containing DNAs were bent more by MutS than complementary sequence DNA (csDNA), did not promote tetramer formation, and allowed MutS conversion to a sliding clamp conformation that eliminated the DNA bends. Addition of second protein responder MutL did not stabilize the MutS-bent forms of DNA. Thus, DNA distortion is only involved at the earliest mispair recognition steps of MMR: MutL does not trap bent DNA conformations, suggesting migrating MutL or MutS/MutL complexes as a conserved feature of MMR. The results promote a mechanism of mismatch DNA bending followed by straightening in initial MutS and MutL responses in MMR. We demonstrate that small angle X-ray scattering with gold labels is an enabling method to examine protein-induced DNA distortions key to the DNA repair, replication, transcription, and packaging. C1 [Hura, Greg L.; Tsai, Chi-Lin; Smith, Jessica M.; Williams, Gareth J.; Alivisatos, A. Paul; Tainer, John A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Claridge, Shelley A.; Smith, Jessica M.; Mastroianni, Alexander J.; Alivisatos, A. Paul] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Mendillo, Marc L.; Putnam, Christopher D.; Kolodner, Richard D.] Ludwig Inst Canc Res, La Jolla, CA 92093 USA. [Putnam, Christopher D.] Univ Calif San Diego, Dept Med, Sch Med, La Jolla, CA 92093 USA. [Kolodner, Richard D.] Univ Calif San Diego, Dept Cellular & Mol Med, Sch Med, La Jolla, CA 92093 USA. [Kolodner, Richard D.] Univ Calif San Diego, Canc Ctr, Sch Med, La Jolla, CA 92093 USA. [Kolodner, Richard D.] Univ Calif San Diego, Inst Genom Med, Sch Med, La Jolla, CA 92093 USA. [Tainer, John A.] Scripps Res Inst, Skaggs Inst Chem Biol, La Jolla, CA 92037 USA. RP Tainer, JA (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM jat@scripps.edu RI Alivisatos , Paul /N-8863-2015 OI Alivisatos , Paul /0000-0001-6895-9048 FU National Institutes of Health (NIH) [P01 CA092584, GM105404]; NIH [GM50006]; Berkeley Laboratory Directed Research and Development funds by the Office of Science, US Department of Energy (DOE); DOE Integrated Diffraction Analysis Technologies program; DOE Office of Science, Basic Energy Sciences [DE-AC02-05CH11231] FX This work was supported by National Institutes of Health (NIH) Structural Cell Biology of DNA Repair Machines Grant P01 CA092584 (to J.A.T. and R. D. K.), by NIH Grant GM50006 (to R. D. K.), and by the Berkeley Laboratory Directed Research and Development funds provided by the Director, Office of Science, US Department of Energy (DOE). The SIBLYS beamline efforts were supported by the DOE Integrated Diffraction Analysis Technologies program and NIH Grant GM105404. The DOE Office of Science, Basic Energy Sciences, Contract DE-AC02-05CH11231, supported A.P.A.'s contribution. NR 54 TC 20 Z9 21 U1 1 U2 21 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD OCT 22 PY 2013 VL 110 IS 43 BP 17308 EP 17313 DI 10.1073/pnas.1308595110 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 238JU UT WOS:000325943300040 PM 24101514 ER PT J AU Han, F Malliakas, CD Stoumpos, CC Sturza, M Claus, H Chung, DY Kanatzidis, MG AF Han, Fei Malliakas, Christos D. Stoumpos, Constantinos C. Sturza, Mihai Claus, Helmut Chung, Duck Young Kanatzidis, Mercouri G. TI Superconductivity and strong intrinsic defects in LaPd1-xBi2 SO PHYSICAL REVIEW B LA English DT Article ID CHARGE-DENSITY-WAVE; GA SQUARE NET; TELLURIUM; LIFEAS; AG; RE; LA; CU AB Two new phases LaPd1-xBi2 and CePd1-xBi2 were obtained by growing single crystals in Bi flux. They adopt the tetragonal ZrCuSi2-type structure and feature Bi-square nets and PbO-type PdBi layers with significant partial Pd occupancy. Bulk superconductivity at 2.1 K and metallic behavior above T-c are observed in LaPd1-xBi2. A small residual resistance ratio (RRR) indicates a strong scattering effect induced by the Pd vacancies, which implies an s-wave pairing symmetry in LaPd1-xBi2. The broadening of the resistivity transition was measured under different magnetic fields demonstrating a high upper critical field of 3 T. Hall effect measurements reveal dominantly electron-like charge carriers and single-band transport behavior in LaPd1-xBi2. The paramagnetic CePd1-xBi2 is nonsuperconducting but shows antiferromagnetic ordering below 6 K. C1 [Han, Fei; Malliakas, Christos D.; Stoumpos, Constantinos C.; Sturza, Mihai; Claus, Helmut; Chung, Duck Young; Kanatzidis, Mercouri G.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Malliakas, Christos D.; Kanatzidis, Mercouri G.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. RP Han, F (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM m-kanatzidis@northwestern.edu RI Han, Fei/N-2021-2013; OI Han, Fei/0000-0001-7782-2713; Stoumpos, Constantinos/0000-0001-8396-9578 FU US Department of Energy, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work is supported by the US Department of Energy, Office of Basic Energy Sciences under Contract No. DE-AC02-06CH11357. NR 53 TC 9 Z9 9 U1 3 U2 56 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 22 PY 2013 VL 88 IS 14 AR 144511 DI 10.1103/PhysRevB.88.144511 PG 6 WC Physics, Condensed Matter SC Physics GA 240IM UT WOS:000326088900003 ER PT J AU Hao, Y Litvinenko, VN Ptitsyn, V AF Hao, Yue Litvinenko, Vladimir N. Ptitsyn, Vadim TI Mitigation of the kink instability in the energy recovery linac based electron-ion collider SO PHYSICAL REVIEW SPECIAL TOPICS-ACCELERATORS AND BEAMS LA English DT Article AB Beam-beam effects in eRHIC, the proposed energy recovery linac (ERL)-based electron-ion collider (EIC) at BNL, have several unique features distinguishing them from those in hadron and lepton colliders. Taking the advantage of the fact that the electron beam is used only once, we expect the luminosity to be 10 times that of a ring-ring collision scheme with similar parameters. However, without instituting proper treatments, the quality of electron and hadron beams can undergo degradation or even beam loss, driven by the beam-beam interactions. Kink instability is one of the most important collective effects of the ion ring due to the special beam-beam interaction in an ERL-based EIC. In this article, we present novel treatments for kink instability in ERL-based EICs including a scheme dedicated to suppressing instability. C1 [Hao, Yue] Brookhaven Natl Lab, Upton, NY 11973 USA. SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. RP Hao, Y (reprint author), Brookhaven Natl Lab, Upton, NY 11973 USA. FU U.S. Department of Energy [DE-AC02-98CH10886] FX The author would like to thank Michael Blaskiewicz and Yun Luo for their constructive help and suggestions. This work is supported by the U.S. Department of Energy under Contract No. DE-AC02-98CH10886. NR 11 TC 1 Z9 1 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-4402 J9 PHYS REV SPEC TOP-AC JI Phys. Rev. Spec. Top.-Accel. Beams PD OCT 22 PY 2013 VL 16 IS 10 AR 101001 DI 10.1103/PhysRevSTAB.16.101001 PG 9 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA 241EQ UT WOS:000326149600001 ER PT J AU Ruegg, A Coh, S Moore, JE AF Rueegg, Andreas Coh, Sinisa Moore, Joel E. TI Corner states of topological fullerenes SO PHYSICAL REVIEW B LA English DT Article ID HGTE QUANTUM-WELLS; INSULATORS; TRANSITION; LATTICE; PARITY AB The unusual electronic properties of the quantum spin Hall or Chern insulator become manifest in the form of robust edge states when samples with boundaries are studied. In this work, we ask if and how the topologically nontrivial electronic structure of these two-dimensional systems can be passed on to their zero-dimensional relatives, namely, fullerenes or other closed-cage molecules. To address this question, we study Haldane's honeycomb lattice model on polyhedral nanosurfaces. We find that for sufficiently large surfaces, characteristic corner states appear for parameters for which the planar model displays a quantized Hall effect. In the electronic structure, these corner states show up as in-gap modes which are well separated from the quasicontinuum of states. We discuss the role of finite-size effects and how the coupling between the corner states lifts the degeneracy in a characteristic way determined by the combined Berry phases which leads to an effective magnetic monopole of charge 2 at the center of the nanosurface. Experimental implications for fullerenes in the large spin-orbit regime are also pointed out. C1 [Rueegg, Andreas; Coh, Sinisa; Moore, Joel E.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Rueegg, Andreas] ETH, CH-8093 Zurich, Switzerland. [Coh, Sinisa; Moore, Joel E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Ruegg, A (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. RI Ruegg, Andreas/B-4498-2010; Moore, Joel/O-4959-2016 OI Moore, Joel/0000-0002-4294-5761 FU Swiss National Science Foundation; Office of Energy Research, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U. S. Department of Energy [DE-AC02-05CH11231]; NSF [DMR-206515] FX A.R. acknowledges collaboration on related projects with C. Lin and F. de Juan and financial support from the Swiss National Science Foundation. S.C. acknowledges discussion with D. Vanderbilt and support by the Director, Office of Energy Research, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U. S. Department of Energy under Contract No. DE-AC02-05CH11231 which provided for the tight-binding calculations. J.E.M. acknowledges financial support from NSF DMR-206515. NR 60 TC 6 Z9 6 U1 2 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 21 PY 2013 VL 88 IS 15 AR 155127 DI 10.1103/PhysRevB.88.155127 PG 11 WC Physics, Condensed Matter SC Physics GA 240HW UT WOS:000326087100007 ER PT J AU Cong, LQ Cao, W Zhang, XQ Tian, Z Gu, JQ Singh, R Han, JG Zhang, WL AF Cong, Longqing Cao, Wei Zhang, Xueqian Tian, Zhen Gu, Jianqiang Singh, Ranjan Han, Jiaguang Zhang, Weili TI A perfect metamaterial polarization rotator SO APPLIED PHYSICS LETTERS LA English DT Article ID TIME-DOMAIN SPECTROSCOPY; TERAHERTZ; POLARIZERS; FILTER; PERFORMANCE AB Polarization conveys valuable information for electromagnetic signal processing exhibiting tremendous potential in developing application driven photonic devices. Manipulation of polarization state of an electromagnetic wave has drawn a lot of research interests in many different fields, especially in the terahertz regime. Here, we propose a unique approach to efficiently rotate the linear polarization of terahertz wave in a broadband configuration with tri-layer metasurfaces. We experimentally observe a nearly perfect orthogonal polarization conversion with an ultrahigh efficiency, demonstrating a ultrathin terahetz rotator. The Fabry-Perot cavity effect in the tri-layer metasurfaces is attributed to the underlying mechanism of high transmittance and polarization rotation. (C) 2013 AIP Publishing LLC. C1 [Cong, Longqing; Zhang, Xueqian; Tian, Zhen; Gu, Jianqiang; Han, Jiaguang; Zhang, Weili] Tianjin Univ, Ctr Terahertz Waves, Tianjin 300072, Peoples R China. [Cong, Longqing; Zhang, Xueqian; Tian, Zhen; Gu, Jianqiang; Han, Jiaguang; Zhang, Weili] Tianjin Univ, Coll Precis Instrument & Optoelect Engn, Tianjin 300072, Peoples R China. [Cao, Wei; Zhang, Weili] Oklahoma State Univ, Sch Elect & Comp Engn, Stillwater, OK 74078 USA. [Singh, Ranjan] Los Alamos Natl Lab, AOT HPE, Los Alamos, NM 87545 USA. RP Han, JG (reprint author), Tianjin Univ, Ctr Terahertz Waves, Tianjin 300072, Peoples R China. EM jiaghan@tju.edu.cn; weili.zhang@okstate.edu RI Singh, Ranjan/B-4091-2010; Zhang, Weili/C-5416-2011; Cong, Longqing/D-1260-2015; Tian, Zhen/D-8707-2015 OI Singh, Ranjan/0000-0001-8068-7428; Zhang, Weili/0000-0002-8591-0200; Cong, Longqing/0000-0003-2839-5940; Tian, Zhen/0000-0002-2861-4325 FU National Science Foundation of China [61007034 61028011, 61138001, 61107085, 61107053]; U.S. National Science Foundation [ECCS-1232081]; Major National Development Project of Scientific Instruments and Equipment [2011YQ150021]; Tianjin Sci-Tech Program [10JCYBJC01400] FX This work was supported by the National Science Foundation of China (Grant Nos. 61007034 61028011, 61138001, 61107085, and 61107053), the U.S. National Science Foundation (Grant No. ECCS-1232081), the Major National Development Project of Scientific Instruments and Equipment (Grant No. 2011YQ150021), and the Tianjin Sci-Tech Program (Grant No. 10JCYBJC01400). NR 26 TC 55 Z9 58 U1 8 U2 79 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD OCT 21 PY 2013 VL 103 IS 17 AR 171107 DI 10.1063/1.4826536 PG 5 WC Physics, Applied SC Physics GA 245HT UT WOS:000326455100007 ER PT J AU Doria, S Yang, N Kumar, A Jesse, S Tebano, A Aruta, C Di Bartolomeo, E Arruda, TM Kalinin, SV Licoccia, S Balestrino, G AF Doria, Sandra Yang, Nan Kumar, Amit Jesse, Stephen Tebano, Antonello Aruta, Carmela Di Bartolomeo, Elisabetta Arruda, Thomas M. Kalinin, Sergei V. Licoccia, Silvia Balestrino, Giuseppe TI Nanoscale mapping of oxygen vacancy kinetics in nanocrystalline Samarium doped ceria thin films SO APPLIED PHYSICS LETTERS LA English DT Article ID NANOMETER RESOLUTION; COMPOSITE MEMBRANES; IONIC-CONDUCTION; TRANSPORT; ELECTROLYTES; PERMEABILITY; MICROSCOPY; DIFFUSION; SURFACES AB The position-dependent oxygen vacancy dynamics induced by a biased scanning probe microscopy tip in Samarium doped ceria thin films grown on MgO (100) substrates is investigated. The granularity of the samples gives rise to spatially dependent local electrochemical activity, as explored by electrochemical strain microscopy. The kinetics of the oxygen vacancy relaxation process is investigated separately for grain boundaries and grains. Higher oxygen vacancy concentration variation and slower diffusion are observed in the grain boundary regions as compared to the grains. (C) 2013 AIP Publishing LLC. C1 [Doria, Sandra; Yang, Nan; Di Bartolomeo, Elisabetta; Licoccia, Silvia] Univ Roma Tor Vergata, NAST Ctr, I-00133 Rome, Italy. [Doria, Sandra] Univ Roma La Sapienza, Dept Phys, I-00185 Rome, Italy. [Yang, Nan; Tebano, Antonello; Aruta, Carmela; Balestrino, Giuseppe] Univ Roma Tor Vergata, CNR SPIN, I-00133 Rome, Italy. [Yang, Nan; Tebano, Antonello; Aruta, Carmela; Balestrino, Giuseppe] Univ Roma Tor Vergata, Dept DICII, I-00133 Rome, Italy. [Kumar, Amit; Jesse, Stephen; Arruda, Thomas M.; Kalinin, Sergei V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Di Bartolomeo, Elisabetta; Licoccia, Silvia] Univ Roma Tor Vergata, Dept Chem Sci & Technol, I-00133 Rome, Italy. RP Aruta, C (reprint author), Univ Roma Tor Vergata, CNR SPIN, I-00133 Rome, Italy. EM carmela.aruta@spin.cnr.it RI Kalinin, Sergei/I-9096-2012; Jesse, Stephen/D-3975-2016; Kumar, Amit/C-9662-2012; Aruta, Carmela/L-2957-2015; OI Kalinin, Sergei/0000-0001-5354-6152; Jesse, Stephen/0000-0002-1168-8483; TEBANO, ANTONELLO/0000-0002-0229-671X; Kumar, Amit/0000-0002-1194-5531; Aruta, Carmela/0000-0002-6917-6667; DI BARTOLOMEO, ELISABETTA/0000-0002-1739-0725 FU META-Materials Enhancement for Technological Applications Project (FP7-PEOPLE-IRSES-Marie Curie Actions) [PIRSES-GA-2010-269182]; Italian MIUR through the FIRB Project [RBAP115AYN]; Division of Scientific User Facilities, U.S. Department of Energy [CNMS2012-016] FX The authors acknowledge META-Materials Enhancement for Technological Applications Project (FP7-PEOPLE-2010-IRSES-Marie Curie Actions, PIRSES-GA-2010-269182) and Italian MIUR through the FIRB Project RBAP115AYN "Oxides at the nanoscale: multifunctionality and applications." The research at ORNL was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Division of Scientific User Facilities, U.S. Department of Energy, in the project CNMS2012-016. NR 32 TC 5 Z9 5 U1 4 U2 47 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD OCT 21 PY 2013 VL 103 IS 17 AR 171605 DI 10.1063/1.4826685 PG 4 WC Physics, Applied SC Physics GA 245HT UT WOS:000326455100018 ER PT J AU Kim, JH Hwang, JH Suh, J Tongay, S Kwon, S Hwang, CC Wu, JQ Park, JY AF Kim, Jong-Hun Hwang, Jin Heui Suh, Joonki Tongay, Sefaattin Kwon, Sangku Hwang, C. C. Wu, Junqiao Park, Jeong Young TI Work function engineering of single layer graphene by irradiation-induced defects SO APPLIED PHYSICS LETTERS LA English DT Article ID MONOLAYER GRAPHENE; RAMAN-SPECTROSCOPY; FORCE MICROSCOPY; EXCITATION; FRICTION; STATES; FILMS; OXIDE AB We report the tuning of electrical properties of single layer graphene by a-beam irradiation. As the defect density increases upon irradiation, the surface potential of the graphene changes, as determined by Kelvin probe force microscopy and Raman spectroscopy studies. X-ray photoelectron spectroscopy studies indicate that the formation of C/O bonding is promoted as the dose of irradiation increases when at atmospheric conditions. Our results show that the surface potential of the graphene can be engineered by introducing atomic-scale defects via irradiation with high-energy particles. (C) 2013 AIP Publishing LLC. C1 [Kim, Jong-Hun; Hwang, Jin Heui; Kwon, Sangku; Park, Jeong Young] Korea Adv Inst Sci & Technol, Ctr Nanomat & Chem React, Inst Basic Sci, Taejon 305701, South Korea. [Kim, Jong-Hun; Hwang, Jin Heui; Kwon, Sangku; Park, Jeong Young] Korea Adv Inst Sci & Technol, Grad Sch EEWS, Taejon 305701, South Korea. [Suh, Joonki; Tongay, Sefaattin; Wu, Junqiao] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Hwang, C. C.] Pohang Univ Sci & Technol POSTECH, PAL, Beamline Res Div, Pohang 790784, South Korea. [Wu, Junqiao] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Park, JY (reprint author), Korea Adv Inst Sci & Technol, Ctr Nanomat & Chem React, Inst Basic Sci, 373-1 Guseong Dong, Taejon 305701, South Korea. EM jeongypark@kaist.ac.kr RI Park, Jeong Young/A-2999-2008; Wu, Junqiao/G-7840-2011 OI Wu, Junqiao/0000-0002-1498-0148 FU IBS (Institute for Basic Science); SRC Centre for Topological Matter through the National Research Foundation (NRF), Republic of Korea [2011-0030787]; Division of Materials Sciences and Engineering of the U.S. Department of Energy [De-Ac02-05Ch11231]; MSIP; POSTECH; [2012R1A2A1A01009249] FX This work was supported by IBS (Institute for Basic Science) and 2012R1A2A1A01009249, and the SRC Centre for Topological Matter (Grant No. 2011-0030787) through the National Research Foundation (NRF), Republic of Korea. The irradiation work and some analyses were supported by the Director, Office of Science, Office of Basic Energy Sciences, and Division of Materials Sciences and Engineering of the U.S. Department of Energy under Contract No. De-Ac02-05Ch11231. Experiments at PLS were supported in part by MSIP and POSTECH. NR 33 TC 38 Z9 38 U1 10 U2 62 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD OCT 21 PY 2013 VL 103 IS 17 AR 171604 DI 10.1063/1.4826642 PG 5 WC Physics, Applied SC Physics GA 245HT UT WOS:000326455100017 ER PT J AU Li, WD Bei, H Tong, Y Dmowski, W Gao, YF AF Li, Weidong Bei, H. Tong, Y. Dmowski, W. Gao, Y. F. TI Structural heterogeneity induced plasticity in bulk metallic glasses: From well-relaxed fragile glass to metal-like behavior SO APPLIED PHYSICS LETTERS LA English DT Article ID RELAXATION AB To reveal the structural origin responsible for the sharp change of the fracture mode on the as-cast and thermally-relaxed status, we use nanomechanical testing to measure the stresses for the onset of plasticity of a metallic glass and develop a stochastic statistical model, which can be used to characterize structural heterogeneity (defect density and strength) inside the metallic glass. Our experiments and calculations found that, with increasing the structural relaxation, the defect density drops by two orders of magnitude. Correspondingly, the fracture of metallic glasses changes from a significantly plastic (metal-like) mode to an extremely brittle (fragile glass) one. (C) 2013 AIP Publishing LLC. C1 [Li, Weidong; Tong, Y.; Dmowski, W.; Gao, Y. F.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Bei, H.; Gao, Y. F.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Bei, H (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. EM Beih@ornl.gov; Ygao7@utk.edu RI Gao, Yanfei/F-9034-2010; OI Gao, Yanfei/0000-0003-2082-857X; Bei, Hongbin/0000-0003-0283-7990 FU U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division; U.S. Department of Energy, Basic Energy Science, Scientific Users Facilities Division FX This work was sponsored by the U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. High energy X-ray diffraction was carried out at the 6-ID beamline, APS, Argonne National Laboratory, supported by U.S. Department of Energy, Basic Energy Science, Scientific Users Facilities Division. We thank the discussion on statistic analysis with Dr. Xiaocun Sun at OIT of University of Tennessee. NR 28 TC 24 Z9 24 U1 4 U2 47 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD OCT 21 PY 2013 VL 103 IS 17 AR 171910 DI 10.1063/1.4827299 PG 5 WC Physics, Applied SC Physics GA 245HT UT WOS:000326455100032 ER PT J AU Lohn, AJ Mickel, PR Marinella, MJ AF Lohn, Andrew J. Mickel, Patrick R. Marinella, Matthew J. TI Dynamics of percolative breakdown mechanism in tantalum oxide resistive switching SO APPLIED PHYSICS LETTERS LA English DT Article ID RELIABILITY; MEMRISTOR; CIRCUIT AB Switching dynamics are studied for tantalum oxide resistive random access memory subjected to long-duration constant current pulses for both SET and RESET transitions. The processes draw parallels to the widely studied percolation model for dielectric breakdown. The RESET transition is shown to consist of changes to critical local conduction sites and their effect on performance parameters such as switching speed and energy are discussed. Additionally, the SET transition shows an unexpected minimum stable resistance state. When driven below that state the device is found to increase resistance, returning to the stable state. (C) 2013 AIP Publishing LLC. C1 [Lohn, Andrew J.; Mickel, Patrick R.; Marinella, Matthew J.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Lohn, AJ (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM ajlohn@sandia.gov FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC0494AL85000] FX The authors would like to acknowledge Robert J. Kaplar and Sandeepan Dasgupta of Sandia National Laboratories for useful discussion regarding dielectric reliability and J. Joshua Yang and Min-Xian Zhang of Hewlett Packard Labs in Palo Alto, CA for their assistance in sample preparation and film deposition. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC0494AL85000. NR 21 TC 11 Z9 11 U1 2 U2 40 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD OCT 21 PY 2013 VL 103 IS 17 AR 173503 DI 10.1063/1.4826277 PG 4 WC Physics, Applied SC Physics GA 245HT UT WOS:000326455100078 ER PT J AU Rajachidambaram, MS Pandey, A Vilayurganapathy, S Nachimuthu, P Thevuthasan, S Herman, GS AF Rajachidambaram, M. S. Pandey, A. Vilayurganapathy, S. Nachimuthu, P. Thevuthasan, S. Herman, G. S. TI Improved stability of amorphous zinc tin oxide thin film transistors using molecular passivation SO APPLIED PHYSICS LETTERS LA English DT Article ID TEMPERATURE FABRICATION; PERFORMANCE; SEMICONDUCTORS AB The role of back channel surface chemistry on amorphous zinc tin oxide (ZTO) bottom gate thin film transistors (TFTs) has been characterized by positive bias-stress measurements and x-ray photoelectron spectroscopy. Positive bias-stress turn-on voltage shifts for ZTO-TFTs were significantly reduced by passivation of back channel surfaces with self-assembled monolayers of n-hexylphosphonic acid when compared to ZTO-TFTs with no passivation. These results indicate that adsorption of molecular species on the exposed back channel of ZTO-TFTs strongly influence observed turn-on voltage shifts, as opposed to charge injection into the dielectric or trapping due to oxygen vacancies. (C) 2013 AIP Publishing LLC. C1 [Rajachidambaram, M. S.; Herman, G. S.] Oregon State Univ, Sch Chem Biol & Environm Engn, Corvallis, OR 97331 USA. [Pandey, A.; Vilayurganapathy, S.; Nachimuthu, P.; Thevuthasan, S.] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99354 USA. RP Herman, GS (reprint author), Oregon State Univ, Sch Chem Biol & Environm Engn, Corvallis, OR 97331 USA. EM greg.herman@oregonstate.edu RI Vilayur Ganapathy, Subramanian/A-1670-2013 FU Oregon Nanoscience and Microtechnologies Institute (ONAMI); Office of Naval Research [200CAR262]; Department of Energy's Office of Biological and Environmental Research FX This work was funded by Oregon Nanoscience and Microtechnologies Institute (ONAMI) and the Office of Naval Research under Contract No. 200CAR262. A portion of the research was performed using EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory (PNNL). Finally, M. S. R. thanks Mr. Jeremy Campbell for providing assistance with UV-Ozone surface treatments, and Ms. Jaana Rajachidambaram and Mr. Brendan Flynn for assistance with XPS peak fitting. NR 34 TC 11 Z9 11 U1 0 U2 17 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD OCT 21 PY 2013 VL 103 IS 17 AR 171602 DI 10.1063/1.4826457 PG 5 WC Physics, Applied SC Physics GA 245HT UT WOS:000326455100015 ER PT J AU Stetsko, YP Shvyd'ko, YV Stephenson, GB AF Stetsko, Yuri P. Shvyd'ko, Yuri V. Stephenson, G. Brian TI Time-delayed beam splitting with energy separation of x-ray channels SO APPLIED PHYSICS LETTERS LA English DT Article ID FREE-ELECTRON LASER; MICHELSON INTERFEROMETER; DIFFRACTION; REFLECTIVITY; DIAMONDS; SILICON; OPTICS; LINE AB We introduce a time-delayed beam splitting method based on the energy separation of x-ray photon beams. It is implemented and theoretically substantiated on an example of an x-ray optical scheme similar to that of the classical Michelson interferometer. The splitter/mixer uses Bragg-case diffraction from a thin diamond crystal. Another two diamond crystals are used as back-reflectors. Because of energy separation and a minimal number (three) of optical elements, the split-delay line has high efficiency and is simple to operate. Due to the high transparency of diamond crystal, the split-delay line can be used in a beam sharing mode at x-ray free-electron laser facilities. (C) 2013 AIP Publishing LLC. C1 [Stetsko, Yuri P.; Shvyd'ko, Yuri V.; Stephenson, G. Brian] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Stetsko, YP (reprint author), Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. EM shvydko@aps.anl.gov FU U.S. Department of Energy, Office of Science [DE-AC02-06CH11357] FX This work was supported by the U.S. Department of Energy, Office of Science, under Contract No. DE-AC02-06CH11357. NR 24 TC 8 Z9 8 U1 0 U2 12 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD OCT 21 PY 2013 VL 103 IS 17 AR 173508 DI 10.1063/1.4826251 PG 4 WC Physics, Applied SC Physics GA 245HT UT WOS:000326455100083 ER PT J AU Hall, AJ Hebert, D Shah, AB Bettge, M Rockett, AA AF Hall, Allen J. Hebert, Damon Shah, Amish B. Bettge, Martin Rockett, Angus A. TI Nanostructured light-absorbing crystalline CuIn(1-x)GaxSe2 thin films grown through high flux, low energy ion irradiation SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID PHYSICAL VAPOR-DEPOSITION; SOLAR-CELLS; PREFERRED ORIENTATION; PRECURSOR FILMS; MICROSTRUCTURE; NONVACUUM; CUINSE2 AB A hybrid effusion/sputtering vacuum system was modified with an inductively coupled plasma (ICP) coil enabling ion assisted physical vapor deposition of CuIn1-xGaxSe2 thin films on GaAs single crystals and stainless steel foils. With <80W rf power to the ICP coil at 620-740 degrees C, film morphologies were unchanged compared to those grown without the ICP. At low temperature (600-670 degrees C) and high rf power (80-400 W), a light absorbing nanostructured highly anisotropic platelet morphology was produced with surface planes dominated by {112}(T) facets. At 80-400W rf power and 640-740 degrees C, both interconnected void and small platelet morphologies were observed while at >270W and above >715 degrees C nanostructured pillars with large inter-pillar voids were produced. The latter appeared black and exhibited a strong {112}(T) texture with interpillar twist angles of +/- 8 degrees. Application of a negative dc bias of 0-50V to the film during growth was not found to alter the film morphology or stoichiometry. The results are interpreted as resulting from the plasma causing strong etching favoring formation of {112}(T) planes and preferential nucleation of new grains, balanced against conventional thermal diffusion and normal growth mechanisms at higher temperatures. The absence of effects due to applied substrate bias suggests that physical sputtering or ion bombardment effects were minimal. The nanostructured platelet and pillar films were found to exhibit less than one percent reflectivity at angles up to 75 degrees from the surface normal. (C) 2013 AIP Publishing LLC. C1 [Hall, Allen J.; Hebert, Damon; Rockett, Angus A.] Univ Illinois, Dept Mat Sci & Engn, Urbana, IL 61801 USA. [Shah, Amish B.] Univ Illinois, Frederick Seitz Mat Res Lab, Ctr Microanal Mat, Urbana, IL 61801 USA. [Bettge, Martin] Argonne Natl Lab, Argonne, IL 60438 USA. RP Hall, AJ (reprint author), Univ Illinois, Dept Mat Sci & Engn, 1304 W Green St, Urbana, IL 61801 USA. EM ahall@illinois.edu RI Rockett, Angus/B-5539-2013 OI Rockett, Angus/0000-0001-9759-8421 NR 33 TC 0 Z9 0 U1 0 U2 4 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD OCT 21 PY 2013 VL 114 IS 15 AR 153505 DI 10.1063/1.4823987 PG 8 WC Physics, Applied SC Physics GA 240SS UT WOS:000326117900017 ER PT J AU Holt, JR Madan, A Harley, ECT Stoker, MW Pinto, T Schepis, DJ Adam, TN Murray, CE Bedell, SW Holt, M AF Holt, Judson R. Madan, Anita Harley, Eric C. T. Stoker, Matt W. Pinto, Teresa Schepis, Dominic J. Adam, Thomas N. Murray, Conal E. Bedell, Stephen W. Holt, Martin TI Observation of semiconductor device channel strain using in-line high resolution X-ray diffraction SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID SILICON AB In-line high resolution X-ray diffraction has been used to analyze embedded silicon-germanium (eSiGe) epitaxially grown in the source/drain regions of complementary metal-oxide-semiconductor devices. Compared to blanket films, the diffraction from patterned devices exhibited distinct features corresponding to the eSiGe in the source/drain regions and Si under the gate and SiGe. The diffraction features modulated with structural changes, alloy composition, and subsequent thermal processing. Reciprocal space measurements taken around the (224) diffraction peak revealed both in-plane (h) and out-of-plane (l) lattice deformation, along with features corresponding to the regular spacing between the gates. (C) 2013 AIP Publishing LLC. C1 [Holt, Judson R.; Madan, Anita; Harley, Eric C. T.; Stoker, Matt W.; Pinto, Teresa; Schepis, Dominic J.] IBM Semicond Res & Dev Ctr, Hopewell Jct, NY 12533 USA. [Adam, Thomas N.] SUNY Albany, Coll Nanoscale Sci & Engn, Albany, NY 12203 USA. [Murray, Conal E.; Bedell, Stephen W.] IBM TJ Watson Res Ctr, Yorktown Hts, NY 10598 USA. [Holt, Martin] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. RP Holt, JR (reprint author), IBM Semicond Res & Dev Ctr, 2050 Route 52, Hopewell Jct, NY 12533 USA. OI Stoker, Matthew/0000-0003-0672-0183 FU U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work was performed at the IBM Semiconductor Research and Development Center (SRDC) 300 mm cleanroom facility in Hopewell Junction, NY. Work done by Martin Holt was supported by the U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 19 TC 7 Z9 7 U1 1 U2 10 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD OCT 21 PY 2013 VL 114 IS 15 AR 154502 DI 10.1063/1.4824819 PG 6 WC Physics, Applied SC Physics GA 240SS UT WOS:000326117900080 ER PT J AU Kuciauskas, D Li, JV Contreras, MA Pankow, J Dippo, P Young, M Mansfield, LM Noufi, R Levi, D AF Kuciauskas, Darius Li, Jian V. Contreras, Miguel A. Pankow, Joel Dippo, Patricia Young, Matthew Mansfield, Lorelle M. Noufi, Rommel Levi, Dean TI Charge carrier dynamics and recombination in graded band gap CuIn1-xGaxSe2 polycrystalline thin-film photovoltaic solar cell absorbers SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID CU(IN,GA)SE-2; EFFICIENCY; LUMINESCENCE; SEMICONDUCTORS; KINETICS; LAYERS AB We report the results of spectroscopic time-resolved photoluminescence (TRPL) analysis for polycrystalline CuIn1-xGaxSe2 (CIGS) films. On the <5 ns time scale, we investigated minority carrier spatial redistribution from the initial absorption profile near the surface of the films to the conduction band minimum. Based on these data, the estimated minority carrier mobility is 75-230 cm(2) V-1 s(-1). Full TRPL decays were analyzed using models for donor-acceptor pair (DAP) recombination. We estimated that the concentration of DAP recombination centers was 5 x 10(15)-10(17) cm(-3). Data also show that Shockley-Reed-Hall and surface recombination are not significant for polycrystalline CIGS absorbers used in high-efficiency photovoltaic solar cells. (C) 2013 AIP Publishing LLC. C1 [Kuciauskas, Darius; Li, Jian V.; Contreras, Miguel A.; Pankow, Joel; Dippo, Patricia; Young, Matthew; Mansfield, Lorelle M.; Noufi, Rommel; Levi, Dean] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Kuciauskas, D (reprint author), Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. RI Li, Jian/B-1627-2016 FU U.S. Department of Energy [DE-AC36-08-GO28308]; National Renewable Energy Laboratory FX This work was supported by the U.S. Department of Energy under Contract No. DE-AC36-08-GO28308 with the National Renewable Energy Laboratory. NR 38 TC 12 Z9 12 U1 0 U2 60 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD OCT 21 PY 2013 VL 114 IS 15 AR 154505 DI 10.1063/1.4825211 PG 6 WC Physics, Applied SC Physics GA 240SS UT WOS:000326117900083 ER PT J AU London, RA Lowry, ME Vernon, SP Stewart, RE AF London, Richard A. Lowry, Mark E. Vernon, Stephen P. Stewart, Richard E. TI Electron cascades in sensors for optical detection of ionizing radiation SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID QUANTUM-WELL STRUCTURES; GAAS; NONLINEARITIES; SEMICONDUCTORS; SPECTROSCOPY; LASERS; INP AB A new class of high-speed detectors, called RadOptic detectors, measures ionizing radiation incident on a transparent semiconductor by sensing changes in the refractive index with an optical probe beam. We describe the role of radiation-initiated electron cascades in setting the sensitivity and the spatial and temporal resolution of RadOptic detectors. We model electron cascades with both analytical and Monte Carlo computational methods. We find that the timescale for the development of an electron cascade is less than of order 100 fs and is not expected to affect the time response of a detector. The characteristic size of the electron cloud is typically less than 2 mu m, enabling high spatial resolution in imaging systems. The electron-hole pair density created by single x-rays is much smaller than the saturation density and, therefore, single events should not saturate the detector. (C) 2013 AIP Publishing LLC. C1 [London, Richard A.; Lowry, Mark E.; Vernon, Stephen P.; Stewart, Richard E.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP London, RA (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Laboratory Directed Research and Development Program at LLNL FX We thank C. Cerjan, A. E. Schach von Wittenau, and P. T. Steele for helpful discussions and L. Chase and H. G. Hughes for help with running MCNP. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344, and was supported by the Laboratory Directed Research and Development Program at LLNL. NR 34 TC 4 Z9 5 U1 0 U2 9 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD OCT 21 PY 2013 VL 114 IS 15 AR 154510 DI 10.1063/1.4825042 PG 8 WC Physics, Applied SC Physics GA 240SS UT WOS:000326117900088 ER PT J AU Pandey, T Singh, DJ Parker, D Singh, AK AF Pandey, Tribhuwan Singh, David J. Parker, David Singh, Abhishek K. TI Thermoelectric properties of beta-FeSi2 SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID SEMICONDUCTING IRON DISILICIDE; ELECTRONIC-STRUCTURE; ELECTRICAL-CONDUCTION; OPTICAL-PROPERTIES; THIN-FILMS; TRANSPORT; FESI2; MECHANISM; LAYERS; CRSI2 AB We investigate the thermoelectric properties of beta-FeSi2 using first principles electronic structure and Boltzmann transport calculations. We report a high thermopower for both p- and n-type beta-FeSi2 over a wide range of carrier concentration and in addition find the performance for n-type to be higher than for the p-type. Our results indicate that, depending upon temperature, a doping level of 3 x 10(20) to 2 x 10(21) cm(-3) may optimize the thermoelectric performance. (C) 2013 AIP Publishing LLC. C1 [Pandey, Tribhuwan; Singh, Abhishek K.] Indian Inst Sci, Mat Res Ctr, Bangalore 560012, Karnataka, India. [Singh, David J.; Parker, David] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Pandey, T (reprint author), Indian Inst Sci, Mat Res Ctr, Bangalore 560012, Karnataka, India. RI Singh, Abhishek/C-2039-2009 OI Singh, Abhishek/0000-0002-7631-6744 FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; D.O.E. Energy Efficiency and Renewable Energy, Vehicle Technologies program FX T.P. acknowledges the hospitality of the Oak Ridge National Laboratory. Work was funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division (T. P., D.J.S., first principles) and the D.O.E. Energy Efficiency and Renewable Energy, Vehicle Technologies program (D.P., analysis). NR 45 TC 7 Z9 7 U1 2 U2 61 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD OCT 21 PY 2013 VL 114 IS 15 AR 153704 DI 10.1063/1.4825217 PG 4 WC Physics, Applied SC Physics GA 240SS UT WOS:000326117900034 ER PT J AU Persaud, A AF Persaud, Arun TI Analysis of slope-intercept plots for arrays of electron field emitters SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID EMISSION PROPERTIES; PARAMETER EXTRACTION; ENHANCEMENT-FACTOR; IONIZATION; CATHODES; CRYSTAL; DRIVEN; FILMS AB In electron field emission experiments, a linear relationship in plots of slope vs. intercept obtained from Fowler-Nordheim analysis is commonly observed for single tips or tip arrays. By simulating samples with many tips, it is shown here that the observed linear relationship results from the distribution of input parameters, assuming a log-normal distribution for the radius of each tip. Typically, a shift from the lower-left to the upper-right of a slope-intercept plot has been correlated with a shift in work function. However, as shown in this paper, the same effect can result from a variation in the number of emitters. (C) 2013 AIP Publishing LLC. C1 EO Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Persaud, A (reprint author), EO Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM APersaud@lbl.gov FU Office of Proliferation Detection (DNN R&D) of the US Department of Energy at the Lawrence Berkeley National Laboratory [DE-AC02-05CHI1231] FX This work was supported by the Office of Proliferation Detection (DNN R&D) of the US Department of Energy at the Lawrence Berkeley National Laboratory under contract number DE-AC02-05CHI1231. NR 34 TC 6 Z9 6 U1 0 U2 6 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD OCT 21 PY 2013 VL 114 IS 15 AR 154301 DI 10.1063/1.4825051 PG 6 WC Physics, Applied SC Physics GA 240SS UT WOS:000326117900067 ER PT J AU Aad, G Abajyan, T Abbott, B Abdallah, J Khalek, SA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Addy, TN Adelman, J Adomeit, S Adye, T Aefsky, S Agatonovic-Jovin, T Aguilar-Saavedra, JA Agustoni, M Ahlen, SP Ahmad, A Ahsan, M Aielli, G Akesson, TPA Akimoto, G Akimov, AV Alam, MA Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alessandria, F Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Aliev, M Alimonti, G Alio, L Alison, J Allbrooke, BMM Allison, LJ Allport, PP Allwood-Spiers, SE Almond, J Aloisio, A Alon, R Alonso, A Alonso, F Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Coutinho, YA Amelung, C Ammosov, VV Dos Santos, SPA Amorim, A Amoroso, S Amram, N Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Anduaga, XS Angelidakis, S Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonaki, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Apolle, R Arabidze, G Aracena, I Arai, Y Arce, ATH Arfaoui, S Arguin, JF Argyropoulos, S Arik, E Arik, M Armbruster, AJ Arnaez, O Arnal, V Arslan, O Artamonov, A Artoni, G Arutinov, D Asai, S Asbah, N Ask, S Asman, B Asquith, L Assamagan, K Astalos, R Astbury, A Atkinson, M Atlay, NB Auerbach, B Auge, E Augsten, K Aurousseau, M Avolio, G Axen, D Azuelos, G Azuma, Y Baak, MA Bacci, C Bach, AM Bachacou, H Bachas, K Backes, M Backhaus, M Mayes, JB Badescu, E Bagiacchi, P Bagnaia, P Bai, Y Bailey, DC Bain, T Baines, JT Baker, OK Baker, S Balek, P Balli, F Banas, E Banerjee, S Banfi, D Bangert, A Bansal, V Bansil, HS Barak, L Baranov, SP Barber, T Barberio, EL Barberis, D Barbero, M Bardin, DY Barillari, T Barisonzi, M Barklow, T Barlow, N Barnett, BM Barnett, RM Baroncelli, A Barone, G Barr, AJ Barreiro, F Da Costa, JBG Bartoldus, R Barton, AE Bartsch, V Basye, A Bates, RL Batkova, L Batley, JR Battistin, M Bauer, F Bawa, HS Beale, S Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, S Beckingham, M Becks, KH Beddall, AJ Beddall, A Bedikian, S Bednyakov, VA Bee, CP Beemster, LJ Beermann, TA Begel, M Belanger-Champagne, C Bell, PJ Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belloni, A Beloborodova, OL Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Benslama, K Bentvelsen, S Berge, D Kuutmann, EB Berger, N Berghaus, F Berglund, E Beringer, J Bernard, C Bernat, P Bernhard, R Bernius, C Bernlochner, FU Berry, T Bertella, C Bertolucci, F Besana, MI Besjes, GJ Bessidskaia, O Besson, N Bethke, S Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Bieniek, SP Bierwagen, K Biesiada, J Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Bittner, B Black, CW Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blazek, T Bloch, I Blocker, C Blocki, J Blum, W Blumenschein, U Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Boddy, CR Boehler, M Boek, J Boek, TT Boelaert, N Bogaerts, JA Bogdanchikov, AG Bogouch, A Bohm, C Bohm, J Boisvert, V Bold, T Boldea, V Bolnet, NM Bomben, M Bona, M Boonekamp, M Bordoni, S Borer, C Borisov, A Borissov, G Borri, M Borroni, S Bortfeldt, J Bortolotto, V Bos, K Boscherinia, D Bosman, M Boterenbrood, H Bouchami, J Boudreau, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boutouil, S Boveia, A Boyd, J Boyko, IR Bozovic-Jelisavcic, I Bracinik, J Branchini, P Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Brazzale, SF Brelier, B Bremer, J Brendlinger, K Brenner, R Bressler, S Bristow, TM Britton, D Brochu, FM Brock, I Brock, R Broggi, F Bromberg, C Bronner, J Brooijmans, G Brooks, T Brooks, WK Brost, E Brown, G Brown, J De Renstrom, PAB Bruncko, D Bruneliere, R Brunet, S Bruni, A Bruni, G Bruschi, M Bryngemark, L Buanes, T Buat, Q Bucci, F Buchanan, J Buchholz, P Buckingham, RM Buckley, AG Buda, SI Budagov, IA Budick, B Buehrer, F Bugge, L Bulekov, O Bundock, AC Bunse, M Buran, T Burckhart, H Burdin, S Burgess, T Burke, S Busato, E Buescher, V Bussey, P Buszello, CP Butler, B Butler, JM Buttar, CM Butterworth, JM Buttinger, W Byszewski, M Urban, SC Caforio, D Cakir, O Calafiura, P Calderini, G Calfayan, P Calkins, R Caloba, LP Caloi, R Calvet, D Calvet, S Toro, RC Camarri, P Cameron, D Caminada, LM Armadans, RC Campana, S Campanelli, M Canale, V Canelli, F Canepa, A Cantero, J Cantrill, R Cao, T Garrido, MDMC Caprini, I Caprini, M Capriotti, D Capua, M Caputo, R Cardarelli, R Carli, T Carlino, G Carminati, L Caron, S Carquin, E Carrillo-Montoya, GD Carter, AA Carter, JR Carvalho, J Casadei, D Casado, MP Caso, C Castaneda-Miranda, E Castelli, A Gimenez, VC Castro, NF Cataldi, G Catastini, P Catinaccio, A Catmore, JR Cattai, A Cattani, G Caughron, S Cavaliere, V Cavalli, D Cavalli-Sforza, M Cavasinni, V Ceradini, F Cerio, B Cerqueira, AS Cerri, A Cerrito, L Cerutti, F Cervelli, A Cetinb, SA Chafaq, A Chakraborty, D Chalupkova, I Chan, K Chang, P Chapleau, B Chapman, JD Chapman, JW Charlton, DG Chavda, V Barajas, CAC Cheatham, S Chekanov, S Chekulaev, SV Chelkov, GA Chelstowska, MA Chen, C Chen, H Chen, S Chen, X Chen, Y Cheng, Y Cheplakov, A El Moursli, RC Chernyatin, V Cheu, E Chevalier, L Chiarella, V Chiefari, G Childers, JT Chilingarov, A Chiodini, G Chisholm, AS Chislett, RT Chitan, A Chizhov, MV Choudalakis, G Chouridou, S Chow, BKB Christidi, IA Christov, A Chromek-Burckhart, D Chu, ML Chudoba, J Ciapetti, G Ciftci, AK Ciftci, R Cinca, D Cindro, V Ciocio, A Cirilli, M Cirkovic, P Citron, ZH Citterio, M Ciubancan, M Clark, A Clark, PJ Clarke, RN Clemens, JC Clement, B Clement, C Coadou, Y Cobal, M Coccaro, A Cochran, J Coelli, S Coffey, L Cogan, JG Coggeshall, J Colas, J Cole, B Cole, S Colijn, AP Collins-Tooth, C Collot, J Colombo, T Colon, G Compostella, G Muino, PC Coniavitis, E Conidi, MC Consonni, SM Consorti, V Constantinescu, S Conta, C Conti, G Conventi, F Cooke, M Cooper, BD Cooper-Sarkar, AM Cooper-Smith, NJ Copic, K Cornelissen, T Corradi, M Corriveau, F Corso-Radu, A Cortes-Gonzalez, A Cortiana, G Costa, G Costa, MJ Costanzo, D Cote, D Cottin, G Courneyea, L Cowan, G Cox, BE Cranmer, K Crepe-Renaudin, S Crescioli, F Ortuzar, MC Cristinziani, M Crosetti, G Cuciuc, CM Almenar, CC Donszelmann, TC Cummings, J Curatolo, M Cuthbert, C Czirr, H Czodrowski, P Czyczula, Z D'Auria, S D'Onofrio, M D'Orazio, A De Sousa, MJDCS Da Via, C Dabrowski, W Dafinca, A Dai, T Dallaire, F Dallapiccola, C Dam, M Damiani, DS Daniells, AC Dao, V Darbo, G Darlea, GL Darmora, S Dassoulas, JA Davey, W David, C Davidek, T Davies, E Davies, M Davignon, O Davison, AR Davygora, Y Dawe, E Dawson, I Daya-Ishmukhametova, RK De, K de Asmundis, R De Castro, S De Cecco, S De Graat, J De Groot, N De Jong, P De la Taille, C De la Torre, H De Lorenzi, F De Nooij, L De Pedis, D De Salvo, A De Sanctis, U De Santo, A De Regie, JBDV De Zorzi, G Dearnaley, WJ Debbe, R Debenedetti, C Dechenaux, B Dedovich, DV Degenhardt, J Del Peso, J Del Prete, T Delemontex, T Deliyergiyev, M Dell'Acqua, A Dell'Asta, L Della Pietra, M della Volpe, D Delmastro, M Delsart, PA Deluca, C Demers, S Demichev, M Demilly, A Demirkoz, B Denisov, SP Derendarz, D Derkaoui, JE Derue, F Dervan, P Desch, K Deviveiros, PO Dewhurst, A DeWilde, B Dhaliwal, S Dhullipudi, R Di Ciaccio, A Di Ciaccio, L Di Donato, C Di Girolamo, A Di Girolamo, B Di Luise, S Di Mattia, A Di Micco, B Di Nardo, R Di Simone, A Di Sipio, R Diaz, MA Diehl, EB Dietrich, J Dietzsch, TA Diglio, S Yagci, KD Dingfelder, J Dinut, F Dionisi, C Dita, P Dita, S Dittus, F Djama, F Djobava, T do Vale, MAB Wemans, ADV Doan, TKO Dobos, D Dobson, E Dodd, J Doglioni, C Doherty, T Dohmae, T Doi, Y Dolejsi, J Dolezal, Z Dolgoshein, BA Donadelli, M Donini, J Dopke, J Doria, A Dos Anjos, 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Zimin, N. I. Zimmermann, C. Zimmermann, R. Zimmermann, S. Zimmermann, S. Zinonos, Z. Ziolkowski, M. Zitoun, R. Zivkovic, L. Zobernig, G. Zoccoli, A. zur Nedden, M. Zurzolo, G. Zutshi, V. Zwalinski, L. CA ATLAS Collaboration TI Search for new phenomena in final states with large jet multiplicities and missing transverse momentum at root s=8 TeV proton-proton collisions using the ATLAS experiment SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering; Jet physics; Supersymmetry; Exotics ID LOCAL SUPERSYMMETRY; GRAND UNIFICATION; SQUARK; SU(5); BOSON; WEAK; LHC AB A search is presented for new particles decaying to large numbers (7 or more) of jets, with missing transverse momentum and no isolated electrons or muons. This analysis uses 20.3 fb(-1) of p p collision data at root s = 8 TeV collected by the ATLAS experiment at the Large Hadron Collider. The sensitivity of the search is enhanced by considering the number of b-tagged jets and the scalar sum of masses of large-radius jets in an event. No evidence is found for physics beyond the Standard Model. The results are interpreted in the context of various simplified supersymmetry-inspired models where gluinos are pair produced, as well as an mSUGRA/CMSSM model. C1 [Jackson, P.; Soni, N.] Univ Adelaide, Sch Chem & Phys, Adelaide, SA, Australia. [Edson, W.; Ernst, J.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Chan, K.; Gingrich, D. M.; Moore, R. W.; Pinfold, J. L.; Saddique, A.; Sbrizzi, A.; Subramania, Hs.; Vaque, F. Vives] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakir, O.; Ciftci, A. K.; Ciftci, R.; Yildiz, H. Duran; Kuday, S.] Ankara Univ, Dept Phys, TR-06100 Ankara, Turkey. [Yilmaz, M.] Gazi Univ, Dept Phys, Ankara, Turkey. [Sultansoy, S.] TOBB Univ Econ & Technol, Div Phys, Ankara, Turkey. 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P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixasa, J. M.] Univ Fed Rio de Janeiro, COPPE EE IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; de Andrade Filho, L. Manhaes] Fed Univ Juiz de Fora UFJF, Juiz De Fora, Brazil. [do Vale, M. A. B.] Fed Univ Sao Joao Del Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadelli, M.; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gadfort, T.; Gibbard, B.; Gordon, H. A.; Hu, X.; Klimentov, A.; Kravchenko, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Metcalfe, J.; Nevski, P.; Okawa, H.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Pleier, M. -A.; Polychronakos, V.; Pravahan, R.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Snyder, S.; Steinberg, P.; Stumer, I.; Takai, H.; Triplett, N.; Undrus, A.; Wenaus, T.; Ye, S.; Zaytsev, A.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Badescu, E.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Cuciuc, C. -M.; Dinut, F.; Dita, P.; Dita, S.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. [Darlea, G. L.] Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Silva, M. L. Gonzalez; Otero y Garzon, G.; Piegaia, R.; Reisin, H.; Romeo, G.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Ask, S.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Buttinger, W.; Carter, J. R.; Chapman, J. D.; French, S. T.; Frost, J. A.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Moeller, V.; Mueller, T.; Parker, M. A.; Robinson, D.; Sandoval, T.; Thomson, M.; Ward, C. P.; Williams, S.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Koffas, T.; Lacey, J.; Marchand, J. F.; McCarthy, T. G.; Oakham, F. G.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Anastopoulos, C.; Andari, N.; Anghinolfi, F.; Avolio, G.; Baak, M. A.; Backes, M.; Banfi, D.; Battistin, M.; Bellomo, M.; Beltramello, O.; Berge, D.; Bogaerts, J. A.; Boyd, J.; Bremer, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Catmore, J. R.; Cattai, A.; Barajas, C. A. Chavez; Childers, J. T.; Chromek-Burckhart, D.; Dell'Acqua, A.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dopke, J.; Dudarev, A.; Duehrssen, M.; Ellis, N.; Elsing, M.; Fabre, C.; Facini, G.; Farthouat, P.; Fassnacht, P.; Franchino, S.; Francis, D.; Froidevaux, D.; Gabaldon, C.; Garonne, V.; Gianotti, F.; Gillberg, D.; Godlewski, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hauschild, M.; Hawkings, R. J.; Heller, M.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Hubacek, Z.; Huhtinen, M.; Jaekel, M. R.; Jansen, H.; Jenni, P.; Jungst, R. M.; Kaneda, M.; Klioutchnikova, T.; Lantzsch, K.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mapelli, L.; Martin, B.; Messina, A.; Meyer, J.; Michal, S.; Molfetas, A.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Negri, G.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Ohm, C. C.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Petersen, J.; Pommes, K.; Poppleton, A.; Poulard, G.; Prasad, S.; Raymond, M.; Rembser, C.; Dos Santos, D. Roda; Roe, S.; Salek, D.; Salzburger, A.; Savu, D. O.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stewart, G. A.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van der Ster, D.; van Eldik, N.; Vandelli, W.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. 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B.; Liu, K.; Liu, M.; Liu, Y.; Peng, H.; Xu, C.; Xu, L.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Yang, H.] Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200030, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Clermont Univ, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Photochim Mol & Macromol Lab, CNRS, IN2P3, F-63177 Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Chen, Y.; Cole, B.; Dodd, J.; Guo, J.; Hu, D.; Hughes, E. W.; Nikiforou, N.; Parsons, J. A.; Penson, A.; Perepelitsa, D. V.; Reale, V. Perez; Scherzer, M. I.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Williams, E.; Willis, W.; Wulf, E.; Zivkovic, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Boelaert, N.; Dam, M.; Galster, G.; Gregersen, K.; Hansen, J. R.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Heisterkamp, S.; Jakobsen, S.; Joergensen, M. D.; Kadlecik, P.; Klinkby, E. B.; Loevschall-Jensen, A. E.; Mackeprang, R.; Mehlhase, S.; Monk, J.; Petersen, T. C.; Pingel, A.; Simonyan, M.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, INFN, Grp Collegato Cosenza, I-87036 Arcavacata Di Rende, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartmento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Grabowska-Bolda, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Blocki, J.; De Renstrom, P. A. Bruckman; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.; Zemla, A.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Cao, T.; Yagci, K. Dindar; Firan, A.; Hoffman, J.; Joffe, D.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Rios, R. R.; Sekula, S. J.; Stroynowski, R.; Wang, H.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Ahsan, M.; Izen, J. M.; Lou, X.; Namasivayam, H.; Reeves, K.; Wong, W. C.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Dassoulas, J. A.; Dietrich, J.; Ferrara, V.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Goebel, M.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Hiller, K. H.; Huettmann, A.; Belenguer, M. Jimenez; Johnert, S.; Katzy, J.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Cavalcanti, T. Perez; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.; Zhu, H.] DESY, Hamburg, Germany. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Dassoulas, J. A.; Dietrich, J.; Ferrara, V.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Goebel, M.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Hiller, K. H.; Huettmann, A.; Belenguer, M. Jimenez; Johnert, S.; Katzy, J.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Cavalcanti, T. Perez; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.; Zhu, H.] DESY, Zeuthen, Germany. [Bunse, M.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Reisinger, I.; Wittig, T.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Czodrowski, P.; Friedrich, F.; Grohs, J. P.; Kobel, M.; Leonhardt, K.; Mader, W. F.; Morgenstern, M.; Prudent, X.; Rudolph, C.; Schnoor, U.; Seifert, F.; Steinbach, P.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B.; Finelli, K. D.; Ko, B. R.; Kotwal, A.; Kruse, M. C.; Li, S.; Liu, M.; Oh, S. H.; Pollard, C. S.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Buckley, A. G.; Clark, P. J.; Debenedetti, C.; Edwards, N. C.; Walls, F. M. Garay; Harrington, R. D.; Korn, A.; Martin, V. J.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Schaelicke, A.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.; Volpi, G.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Aad, G.; Amoroso, S.; Barber, T.; Bernhard, R.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Christov, A.; Consorti, V.; Di Simone, A.; Fehling-Kaschek, M.; Flechl, M.; Giuliani, C.; Hartert, J.; Herten, G.; Jakobs, K.; Koeneke, K.; Kuehn, S.; Lai, S.; Landgraf, U.; Lohwasser, K.; Ludwig, I.; Ludwig, J.; Madar, R.; Mahboubi, K.; Mohr, W.; Parzefall, U.; Rammensee, M.; Rave, T. C.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Siegert, F.; Stoerig, K.; Sundermann, J. E.; Temming, K. K.; Thoma, S.; Tsiskaridze, V.; Ungaro, F. C.; Venturi, M.; Vivarelli, I.; von Radziewski, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Winkelmann, S.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Alexandre, G.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Bucci, F.; Toro, R. Camacho; Clark, A.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Latour, B. Martin Dit; Mermod, P.; Herrera, C. Mora; Muenstermann, D.; Nektarijevic, S.; Nikolics, K.; Pasztor, G.; Picazio, A.; Pohl, M.; Rosbach, K.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Beccherle, R.; Caso, C.; Darbo, G.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Univ Genoa, Ist Nazl Fis Nucl, Sez Genova, Genoa, Italy. [Barberis, D.; Caso, C.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Khubua, J.; Mchedlidze, G.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Bussey, P.; Buttar, C. M.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Quilty, D.; Ravenscroft, T.; Robson, A.; Saxon, D. H.; Smith, K. M.; St. Denis, R. D.; Steele, G.; Thompson, A. S.; Wraight, K.; Wright, M.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bierwagen, K.; Blumenschein, U.; Brandt, O.; Evangelakou, D.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Hensel, C.; Kawamura, G.; Keil, M.; Knue, A.; Kohn, F.; Krieger, N.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Meyer, J.; Morel, J.; Nackenhorst, O.; Pashapour, S.; Peters, R. F. Y.; Quadt, A.; Roe, A.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Schroeder, T. Vazquez; Weingarten, J.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Brown, J.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] Univ Grenoble 1, Lab Phys Subatom & Cosmol, Grenoble, France. [Albrand, S.; Brown, J.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] CNRS, IN2P3, Grenoble, France. [Albrand, S.; Brown, J.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] Inst Natl Polytech Grenoble, F-38031 Grenoble, France. [Addy, T. N.; Harvey, A.; McFarlane, K. W.; Shin, T.; Vassilakopoulos, V. I.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Da Costa, J. Barreiro Guimaraes; Belloni, A.; Butler, B.; Catastini, P.; Conti, G.; Franklin, M.; Huth, J.; Jeanty, L.; Mateos, D. Lopez; Mercurio, K. M.; Mills, C.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Yen, A. L.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Anders, G.; Andrei, V.; Davygora, Y.; Dietzsch, T. A.; Dunford, M.; Hanke, P.; Hofmann, J. I.; Khomich, A.; Kluge, E. -E.; Laier, H.; Lang, V. S.; Lendermann, V.; Meier, K.; Mueller, F.; Poddar, S.; Scharfa, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Kugel, A.; Schroer, N.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Franz, S.; Jussel, P.; Kneringer, E.; Lukas, W.; Nagai, K.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Cinca, D.; Gandrajula, R. P.; Halladjian, G.; Limper, M.; Mallik, U.; Mandrysch, R.; Morange, N.; Pylypchenko, Y.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Ruiz-Martinez, A.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Aleksandrov, I. N.; Bardin, D. Y.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Grigalashvili, N.; Huseynov, N.; Karpov, S. N.; Kazarinov, M. Y.; Kharchenko, D.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rumyantsev, L.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.; Zimin, N. I.] Joint Inst Nucl Res Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Arai, Y.; Doi, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Mitsui, S.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [King, M.; Kishimoto, T.; Kitamura, T.; Kurashige, H.; Matsushita, T.; Ochi, A.; Shimizu, S.; Takeda, H.; Tani, K.; Watanabe, I.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Sasao, N.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Verzini, M. J. Alconada; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Verzini, M. J. Alconada; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Allison, L. J.; Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Bianco, M.; Cataldi, G.; Chiodini, G.; Gorini, E.; Grancagnolo, F.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Univ Salento, Ist Nazl Fis Nucl, Sez Lecce, Lecce, Italy. [Bianco, M.; Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Greenshaw, T.; Gwilliam, C. B.; Hayward, H. S.; Jackson, J. N.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Schnellbach, Y. J.; Sellers, G.; Vossebeld, J. H.; Waller, P.; Wrona, B.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia. [Bona, M.; Carter, A. A.; Cerrito, L.; Eisenhandler, E.; Ellis, K.; Fletcher, G.; Goddard, J. R.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Rizvi, E.; Salamanna, G.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Alam, M. A.; Berry, T.; Boisvert, V.; Brooks, T.; Cantrill, R.; Cooper-Smith, N. J.; Cowan, G.; Duguid, L.; Edwards, C. A.; George, S.; Gibson, S. M.; Goncalo, R.; Vazquez, J. G. Panduro; Pastore, Fr.; Rose, M.; Spano, F.; Strong, J. A.; Teixeira-Dias, P.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Baker, S.; Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christidi, I. A.; Cooper, B. D.; Davison, A. R.; Dobson, E.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Lambourne, L.; Nash, M.; Nurse, E.; Ochoa, M. I.; Pilkington, A. D.; Prabhu, R.; Sherwood, P.; Simmons, B.; Taylor, C.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Bernius, C.; Dhullipudi, R.; Greenwood, Z. D.; Sawyer, L.; Sircar, A.; Subramaniam, R.; Tamsett, M. C.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Jarlskog, G.; Lytken, E.; Meirose, B.; Mjoernmark, J. U.; Smirnova, O.; Wielers, M.] Lund Univ, Fysiska Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Labarga, L.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Arnaez, O.; Blum, W.; Buescher, V.; Caputo, R.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Goeringer, C.; Handel, C.; Heck, T.; Hohlfeld, M.; Hsu, P. J.; Huelsing, T. A.; Ji, W.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Meyer, C.; Moreno, D.; Moritz, S.; Mueller, T.; Neusiedl, A.; Poettgen, R.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Almond, J.; Borri, M.; Brown, G.; Chavda, V.; Cox, B. E.; Da Via, C.; Forti, A.; Howarth, J.; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Marx, M.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Robinson, J. E. M.; Tomlinson, L.; Watts, S.; Woudstra, M. J.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Alio, L.; Barbero, M.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Nagai, Y.; Odier, J.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Alio, L.; Barbero, M.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Nagai, Y.; Odier, J.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Brau, B.; Colon, G.; Dallapiccola, C.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Dufour, M-A.; Klemetti, M.; Mantifel, R.; Robertson, S. H.; Schram, M.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Diglio, S.; Hamano, K.; Jennens, D.; Kubota, T.; Limosani, A.; Hanninger, G. Nunes; Phan, A.; Shao, Q. T.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Volpi, M.; White, M. J.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Armbruster, A. J.; Chapman, J. W.; Chelstowska, M. A.; Cirilli, M.; Dai, T.; Diehl, E. B.; Dubbert, J.; Feng, H.; Ferretti, C.; Goldfarb, S.; Harper, D.; Levin, D.; Li, X.; Liu, L.; Mc Kee, S. P.; Neal, H. A.; Panikashvili, N.; Qian, J.; Scheirich, D.; Searcy, J.; Thun, R. P.; Walch, S.; Wilson, A.; Wooden, G.; Wu, Y.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Hauser, R.; Hayden, D.; Holzbauer, J. L.; Huston, J.; Koll, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schwienhorst, R.; Stelzer, H. J.; Tollefson, K.; True, P.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alessandria, F.; Alimonti, G.; Andreazza, A.; Besana, M. I.; Broggi, F.; Carminati, L.; Cavalli, D.; Citterio, M.; Coelli, S.; Consonni, S. M.; Costa, G.; Fanti, M.; Favareto, A.; Giugni, D.; Koletsou, I.; Lari, T.; Mandelli, L.; Mazzanti, M.; Meloni, F.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Rivoltella, G.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Volpini, G.] Univ Milan, INFN, Sez Milano, Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Favareto, A.; Meloni, F.; Perini, L.; Pizio, C.; Ragusa, F.; Rivoltella, G.; Simoniello, R.; Turra, R.] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Satsounkevitch, I.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Asbah, N.; Azuelos, G.; Bouchami, J.; Dallaire, F.; Davies, M.; Gauthier, L.; Giunta, M.; Leroy, C.; Martin, J. P.; Rezvani, R.; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.] Acad Sci, PN Lebedev Inst Phys, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.] Moscow Engn Phys Inst MEPhI, Moscow, Russia. [Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Beale, S.; Becker, S.; Biebel, O.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; De Graat, J.; Duckeck, G.; Ebke, J.; Elmsheuser, J.; Engl, A.; Galea, C.; Heller, C.; Hertenberger, R.; Legger, F.; Lorenz, J.; Mann, A.; Meineck, C.; Nunnemann, T.; Oakes, L. B.; Rauscher, F.; Reznicek, P.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Schieck, J.; Schmitt, C.; Staude, A.; Vladoiu, D.; Walker, R.; Will, J. Z.; Wittkowski, J.; Zibell, A.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bittner, B.; Bronner, J.; Capriotti, D.; Compostella, G.; Cortiana, G.; Flowerdew, M. J.; Giovannini, P.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kotov, S.; Kroha, H.; Macchiolo, A.; Manfredini, A.; Menke, S.; Moser, H. G.; Nagel, M.; Nisius, R.; Oberlack, H.; Pahl, C.; Pospelov, G. E.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Stern, S.; Stonjek, S.; Vanadia, M.; von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; della Volpe, D.; Di Donato, C.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Patricelli, S.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Univ Naples Federico II, INFN, Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Chiefari, G.; della Volpe, D.; Di Donato, C.; Giordano, R.; Merola, L.; Patricelli, S.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Sci Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Dao, V.; De Groot, N.; Filthaut, F.; Klok, P. F.; Koenig, A. C.; Raas, M.; Salvucci, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Castelli, A.; Colijn, A. P.; De Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Oussoren, K. P.; Pani, P.; Ruckstuhl, N.; Ta, D.; Tsiakiris, M.; Valencic, N.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Castelli, A.; Colijn, A. P.; De Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Oussoren, K. P.; Pani, P.; Ruckstuhl, N.; Ta, D.; Tsiakiris, M.; Valencic, N.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Univ Amsterdam, Amsterdam, Netherlands. [Calkins, R.; Chakraborty, D.; Cole, S.; De Lima, J. G. Rocha; Suhr, C.; Yurkewicz, A.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL USA. [Anisenkov, A. V.; Beloborodova, O. L.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Skovpen, K. Yu.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Budick, B.; Cranmer, K.; Haas, A.; van Huysduynen, L. Hooft; Kaplan, B.; Konoplich, R.; Krasznahorkay, A.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.; Prokofiev, K.] NYU, Dept Phys, New York, NY 10003 USA. [Fisher, M. J.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Strang, M.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Gutierrez, P.; Jana, D. K.; Marzin, A.; Meera-Lebbai, R.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Snow, J.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Khanov, A.; Rizatdinova, F.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Hamal, P.; Hrabovsky, M.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Brost, E.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Reinsch, A.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Auge, E.; Binet, S.; Bourdarios, C.; De la Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Teinturier, M.; Tran, H. L.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Ahmad, A.; Auge, E.; Binet, S.; Bourdarios, C.; De la Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Teinturier, M.; Tran, H. L.; Zerwas, D.; Zhang, Z.] CNRS, IN2P3, F-91405 Orsay, France. [Hanagaki, K.; Hirose, M.; Lee, J. S. H.; Nomachi, M.; Okamura, W.; Sugaya, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Buran, T.; Cameron, D.; Gjelsten, B. K.; Gramstad, E.; Lund, E.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Read, A. L.; Rohne, O.; Smestad, L.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Apolle, R.; Barr, A. J.; Boddy, C. R.; Buchanan, J.; Buckingham, R. M.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; King, R. S. B.; Kogan, L. A.; Larner, A.; Lewis, A.; Liang, Z.; Livermore, S. S. A.; Mattravers, C.; Nickerson, R. B.; Pachal, K.; Pinder, A.; Robichaud-Veronneau, A.; Ryder, N. C.; Sawyer, C.; Short, D.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Young, C. J. S.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Colombo, T.; Conta, C.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Univ Pavia, INFN, Sez Pavia, I-27100 Pavia, Italy. [Colombo, T.; Conta, C.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Degenhardt, J.; Fratina, S.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Keener, P. T.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Marshall, Z.; Newcomer, F. M.; Olivito, D.; Ospanov, R.; Reece, R.; Saxon, J.; Schaefer, D.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Van Berg, R.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dotti, A.; Giannetti, P.; Roda, C.; Sarri, F.; White, S.; Zinonos, Z.] Univ Pisa, INFN, Sez Pisa, Pisa, Italy. [Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dotti, A.; Giannetti, P.; Roda, C.; Sarri, F.; White, S.; Zinonos, Z.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Escobar, C.; Kittelmann, T.; Mueller, J.; Prieur, D.; Sapp, K.; Savinov, V.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Dos Santos, S. P. Amor; Amorim, A.; Anjos, N.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Wemans, A. Do Valle; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Jorge, P. M.; Lopes, L.; Miguens, J. Machado; Maio, A.; Maneira, J.; Marques, C. N.; Oliveira, M.; Onofre, A.; Palma, A.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] LIP, Lab Instrumentacao & Fis Expt Particulas, P-1000 Lisbon, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. [Bohm, J.; Chudoba, J.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Myska, M.; Nemecek, S.; Ruzicka, P.; Schovancova, J.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Tic, T.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Gallus, P.; Gunther, J.; Jakubek, J.; Kohout, Z.; Kral, V.; Pospisil, S.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solar, M.; Solc, J.; Sopko, V.; Sopko, B.; Stekl, I.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Torregrosa, E. Fullana; Kodys, P.; Leitner, R.; Novakova, J.; Pleskot, V.; Rybar, M.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.; Wilhelm, I.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Ammosov, V. V.; Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Ivashin, A. V.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] Inst High Energy Phys, State Res Ctr, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Gillman, A. R.; Haywood, S. J.; Kirk, J.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Tyndel, M.; Wickens, F. J.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Benslama, K.] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Pedis, D.; De Salvo, A.; De Zorzi, G.; Dionisi, C.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Rossi, E.; Tehrani, F. Safai; Sidoti, A.; Camillocci, E. Solfaroli; Vari, R.; Veneziano, S.; Zanello, L.] Univ Roma La Sapienza, INFN, Sez Roma 1, I-00185 Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Zorzi, G.; Dionisi, C.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Rossi, E.; Camillocci, E. Solfaroli; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Liberti, B.; Marchese, F.; Mazzaferro, L.; Salamon, A.; Santonico, R.] Univ Roma Tor Vergata, INFN, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Cattani, G.; Di Ciaccio, A.; Marchese, F.; Mazzaferro, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Branchini, P.; Ceradini, F.; Di Luise, S.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Stanescu, C.; Trovatelli, M.] Univ Roma Tre, INFN, Sez Roma Tre, Rome, Italy. [Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Luise, S.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.; Lablak, S.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA Marrakech, Fac Sci Semlalia, Marrakech, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Abreu, H.; Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Bolnet, N. M.; Boonekamp, M.; Chevalier, L.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Grabas, H. M. X.; Guyot, C.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Legendre, M.; Maiani, C.; Mal, P.; Ramos, J. A. Manjarres; Mansoulie, B.; Martinez, H.; Meric, N.; Meyer, J-P.; Mijovic, L.; Hong, V. Nguyen Thi; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Resende, B.; Royon, C. R.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.; Tsionou, D.; Vranjes, N.; Xiao, M.] CEA Saclay Commissariat Energie Atom & Energies A, DSM IRFU, Inst Rech Lois Fondamentales Univers, Gif Sur Yvette, France. [Damiani, D. S.; Grillo, A. A.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Mitrevski, J.; Nielsen, J.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Beckingham, M.; Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Hsu, S. -C.; Keller, J. S.; Lubatti, H. J.; Rompotis, N.; Rothberg, J.; Verducci, M.; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Paredes, B. Lopez; Mcfayden, J. A.; Miyagawa, P. S.; Owen, S.; Paganis, E.; Suruliz, K.; Tovey, D. R.; Tua, A.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Ibragimov, I.; Ikematsu, K.; Rammes, M.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Dawe, E.; Godfrey, J.; Kvita, J.; O'Neil, D. C.; Petteni, M.; Stelzer, B.; Tanasijczuk, A. J.; Trottier-McDonald, M.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Mayes, J. Backus; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Hansson, P.; Kagan, M.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nelson, T. K.; Piacquadio, G.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Strauss, E.; Su, D.; Swiatlowski, M.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Batkova, L.; Blazek, T.; Federic, P.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Ferencei, J.; Kladiva, E.; Seman, M.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Carrillo-Montoya, G. D.; Leney, K. J. C.; Garcia, B. R. Mellado; Quayle, W. B.; Ruan, X.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Asman, B.; Bendtz, K.; Bessidskaia, O.; Bohm, C.; Clement, C.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Holmgren, S. O.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Papadelis, A.; Petridis, A.; Plucinski, P.; Silverstein, S. B.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Asman, B.; Bendtz, K.; Bessidskaia, O.; Clement, C.; Gellerstedt, K.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Petridis, A.; Plucinski, P.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Ahmad, A.; Arfaoui, S.; DeWilde, B.; Engelmann, R.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Puldon, D.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Ahmad, A.; Arfaoui, S.; DeWilde, B.; Engelmann, R.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Puldon, D.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Bartsch, V.; De Santo, A.; Martin-Haugh, S.; Potter, C. J.; Rose, A.; Salvatore, F.; Castillo, I. Santoyo; Sutton, M. R.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Bangert, A.; Black, C. W.; Cuthbert, C.; Jeng, G. -Y.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Waugh, A. T.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Chu, M. L.; Hou, S.; Jamin, D. O.; Lee, C. A.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; Mazini, R.; Ren, Z. L.; Soh, D. A.; Teng, P. K.; Wang, J.; Wang, S. M.; Weng, Z.; Zhang, L.] Acad Sinica, Inst Phys, Taipei 115, Taiwan. [Di Mattia, A.; Kajomovitz, E.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; Vallecorsa, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Bella, G.; Benary, O.; Benhammou, Y.; Etzion, E.; Gershon, A.; Gueta, O.; Guttman, N.; Munwes, Y.; Oren, Y.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkialas, I.; Iliadis, D.; Kordas, K.; Kouskoura, V.; Nomidis, I.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Ishitsuka, M.; Jinnouchi, O.; Kanno, T.; Kuze, M.; Nagai, R.; Nobe, T.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Bailey, D. C.; Brelier, B.; Farooque, T.; Fatholahzadeh, B.; Ilic, N.; Keung, J.; Krieger, P.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Spreitzer, T.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Canepa, A.; Chekulaev, S. V.; Fortin, D.; Koutsman, A.; Losty, M. J.; Oram, C. J.; Codina, E. Perez; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Bustos, A. C. Florez; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Kurata, M.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Napier, A.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Loureiro, K. F.; Navas, L. Mendoza; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Farrell, S.; Gerbaudo, D.; Eschrich, I. Gough; Lankford, A. J.; Magnoni, L.; Mete, A. S.; Nelson, A.; Rao, K.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Taffard, A.; Toggerson, B.; Unel, G.; Werth, M.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Pinamonti, M.; Shaw, K.; Soualah, R.] Univ Udine, INFN, Grp Collegato Udine, I-33100 Udine, Italy. [Acharya, B. S.] Univ Udine, ICTP, Trieste, Italy. [Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Shaw, K.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Coggeshall, J.; Errede, D.; Errede, S.; Lie, K.; Liss, T. M.; McCarn, A.; Neubauer, M. S.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Brenner, R.; Buszello, C. P.; Coniavitis, E.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Pelikan, D.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; March, L.; Moya, M. Minano; Llacer, M. Moreno; Garcia, E. Oliver; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Sanchez, J.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] CSIC, Valencia, Spain. [Axen, D.; Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Loh, C. W.; Mills, W. J.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Astbury, A.; Bansal, V.; Berghaus, F.; Bernlochner, F. U.; Courneyea, L.; David, C.; Fincke-Keeler, M.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Lessard, J-R.; Marino, C. P.; Martyniuk, A. C.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Farrington, S. M.; Janus, M.; Jeske, C.; Jones, G.; Martin, T. A.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Kimura, N.; Mitani, T.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Alon, R.; Barak, L.; Bressler, S.; Citron, Z. H.; Duchovni, E.; Gabizon, O.; Gross, E.; Groth-Jensen, J.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Milstein, D.; Roth, I.; Silbert, O.; Smakhtin, V.; Vitells, O.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw; Castaneda-Miranda, E.; Chen, X.; Dos Anjos, A.; Castillo, L. R. Flores; Gutzwiller, O.; Hard, A. S.; Jared, R. C.; Ji, H.; Ju, X.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Morales, M. I. Pedraza; Sarangi, T.; Wang, H.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Fleischmann, P.; Redelbach, A.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.] Julius Maximilians Univ, Fak Phys & Astron, Wurzburg, Germany. [Barisonzi, M.; Becks, K. H.; Beermann, T. A.; Boek, J.; Boek, T. T.; Braun, H. M.; Cornelissen, T.; Duda, D.; Fischer, J.; Fleischmann, S.; Flick, T.; Gorfine, G.; Hamacher, K.; Harenberg, T.; Hirschbuehl, D.; Kalinin, S.; Kersten, S.; Khoroshilov, A.; Kohlmann, S.; Lenzen, G.; Maettig, P.; Mechtel, M.; Neumann, M.; Pataraia, S.; Sandhoff, M.; Sartisohn, G.; Sturm, P.; Wagner, W.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany. [Adelman, J.; Baker, O. K.; Bedikian, S.; Almenar, C. Cuenca; Cummings, J.; Czyczula, Z.; Demers, S.; Erdmann, J.; Garberson, F.; Golling, T.; Guest, D.; Henrichs, A.; Lagouri, T.; Lee, L.; Leister, A. G.; Loginov, A.; Tipton, P.; Wall, R.; Walsh, B.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Becker, K.; Rahal, G.] IN2P3, Ctr Calcul Inst Natl Phys Nucl & Phys Particules, Villeurbanne, France. [Acharya, B. S.] Kings Coll London, Dept Phys, London, England. [Aguilar-Saavedra, J. A.] LIP, Lab Instrumentacao & Fis Expt Particulas, P-1000 Lisbon, Portugal. [Amorim, A.; Gomes, A.; Maio, A.; Pina, J.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amorim, A.; Gomes, A.; Maio, A.; Pina, J.] Univ Lisbon, CFNUL, P-1699 Lisbon, Portugal. [Apolle, R.; Davies, E.; Mattravers, C.; Nash, M.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Azuelos, G.; Gingrich, D. M.; Oakham, F. G.; Savard, P.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Bawa, H. S.; Gao, Y. S.; Lowe, A. J.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beloborodova, O. L.; Maximov, D. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Carvalho, J.; Fiolhais, M. C. N.; Oliveira, M.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Demirkoz, B.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Dhullipudi, R.; Greenwood, Z. D.; Sawyer, L.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Wemans, A. Do Valle] Univ Nova Lisboa, Dep Fis, Caparica, Portugal. [Wemans, A. Do Valle] Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Ge, P.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Gkialas, I.; Papageorgiou, K.] Univ Aegean, Dept Financial & Management Engn, Chios, Greece. [Grinstein, S.; Rozas, A. Juste; Martinez, M.] ICREA, Barcelona, Spain. [Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Huseynov, N.] Azerbaijan Acad Sci, Inst Phys, Baku 370143, Azerbaijan. [Kono, T.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo 112, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Li, B.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Liang, Z.; Soh, D. A.; Weng, Z.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou, Peoples R China. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Liu, K.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Liu, K.] Univ Paris Diderot, Paris, France. [Liu, K.] CNRS, IN2P3, Paris, France. [Mal, P.; Talyshev, A. A.] Natl Inst Sci Educ & Res, Sch Phys Sci, Bhubaneswar, Orissa, India. [Messina, A.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Mountricha, E.; Xu, C.] CEA Saclay Commissariat Energie Atom & Energies A, DSM IRFU Inst Rech Lois Fondamentales Univers, Gif Sur Yvette, France. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys, Dolgoprudnyi, Russia. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Technol State Univ, Dolgoprudnyi, Russia. [Nessi, M.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Nessi, M.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Pasztor, G.; Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Peters, R. F. Y.] DESY, Hamburg, Germany. [Peters, R. F. Y.] DESY, Zeuthen, Germany. [Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Spousta, M.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Tamsett, M. C.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Tikhomirov, V. O.] Moscow Engn & Phys Inst MEPhI, Moscow, Russia. [Vickey, T.] Univ Oxford, Dept Phys, Oxford, England. [Wildt, M. A.] Univ Hamburg, Inst Expt Phys, Hamburg, Germany. [Xu, L.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. RP Aad, G (reprint author), Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. RI de Groot, Nicolo/A-2675-2009; Hejbal, Jiri/H-1358-2014; Marcisovsky, Michal/H-1533-2014; Mikestikova, Marcela/H-1996-2014; Lysak, Roman/H-2995-2014; Tomasek, Lukas/G-6370-2014; Svatos, Michal/G-8437-2014; Chudoba, Jiri/G-7737-2014; Peleganchuk, Sergey/J-6722-2014; Bosman, Martine/J-9917-2014; Castro, Nuno/D-5260-2011; Grinstein, Sebastian/N-3988-2014; Wemans, Andre/A-6738-2012; Robson, Aidan/G-1087-2011; Kuday, Sinan/C-8528-2014; Smirnova, Oxana/A-4401-2013; Gabrielli, Alessandro/H-4931-2012; Zimmermann, Claus/E-9598-2014; Fabbri, Laura/H-3442-2012; Villa, Mauro/C-9883-2009; Nozka, Libor/G-5550-2014; Nemecek, Stanislav/G-5931-2014; Kepka, Oldrich/G-6375-2014; Lokajicek, Milos/G-7800-2014; Jakoubek, Tomas/G-8644-2014; Staroba, Pavel/G-8850-2014; Kupco, Alexander/G-9713-2014; Solfaroli Camillocci, Elena/J-1596-2012; Lee, Jason/B-9701-2014; Livan, Michele/D-7531-2012; Boyko, Igor/J-3659-2013; Brooks, William/C-8636-2013; Moraes, Arthur/F-6478-2010; Ferrando, James/A-9192-2012; Snesarev, Andrey/H-5090-2013; Warburton, Andreas/N-8028-2013; Turchikhin, Semen/O-1929-2013; Sukharev, Andrey/A-6470-2014; Doyle, Anthony/C-5889-2009; Fassi, Farida/F-3571-2016; la rotonda, laura/B-4028-2016; Monzani, Simone/D-6328-2017; Grancagnolo, Francesco/K-2857-2015; Korol, Aleksandr/A-6244-2014; Karyukhin, Andrey/J-3904-2014; Capua, Marcella/A-8549-2015; Tartarelli, Giuseppe Francesco/A-5629-2016; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Olshevskiy, Alexander/I-1580-2016; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; KHODINOV, ALEKSANDR/D-6269-2015; O'Shea, Val/G-1279-2010; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Yang, Haijun/O-1055-2015; Andreazza, Attilio/E-5642-2011; Carvalho, Joao/M-4060-2013; Demirkoz, Bilge/C-8179-2014; Mashinistov, Ruslan/M-8356-2015; Buttar, Craig/D-3706-2011; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Hansen, John/B-9058-2015; Grancagnolo, Sergio/J-3957-2015; spagnolo, stefania/A-6359-2012; Ciubancan, Liviu Mihai/L-2412-2015; Shmeleva, Alevtina/M-6199-2015; Camarri, Paolo/M-7979-2015; Gavrilenko, Igor/M-8260-2015; Akimov, Andrey/N-1769-2015; Tikhomirov, Vladimir/M-6194-2015; Chekulaev, Sergey/O-1145-2015; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; Gutierrez, Phillip/C-1161-2011; Ventura, Andrea/A-9544-2015; De, Kaushik/N-1953-2013; Mitsou, Vasiliki/D-1967-2009; White, Ryan/E-2979-2015; Joergensen, Morten/E-6847-2015; Riu, Imma/L-7385-2014; Mir, Lluisa-Maria/G-7212-2015; Della Pietra, Massimo/J-5008-2012; Cavalli-Sforza, Matteo/H-7102-2015; Petrucci, Fabrizio/G-8348-2012; Negrini, Matteo/C-8906-2014; Ferrer, Antonio/H-2942-2015 OI Mikestikova, Marcela/0000-0003-1277-2596; Tomasek, Lukas/0000-0002-5224-1936; Svatos, Michal/0000-0002-7199-3383; Peleganchuk, Sergey/0000-0003-0907-7592; Bosman, Martine/0000-0002-7290-643X; Castro, Nuno/0000-0001-8491-4376; Grinstein, Sebastian/0000-0002-6460-8694; Wemans, Andre/0000-0002-9669-9500; Kuday, Sinan/0000-0002-0116-5494; Smirnova, Oxana/0000-0003-2517-531X; Gabrielli, Alessandro/0000-0001-5346-7841; Fabbri, Laura/0000-0002-4002-8353; Villa, Mauro/0000-0002-9181-8048; Solfaroli Camillocci, Elena/0000-0002-5347-7764; Lee, Jason/0000-0002-2153-1519; Livan, Michele/0000-0002-5877-0062; Boyko, Igor/0000-0002-3355-4662; Brooks, William/0000-0001-6161-3570; Moraes, Arthur/0000-0002-5157-5686; Ferrando, James/0000-0002-1007-7816; Warburton, Andreas/0000-0002-2298-7315; Turchikhin, Semen/0000-0001-6506-3123; Doyle, Anthony/0000-0001-6322-6195; Veloso, Filipe/0000-0002-5956-4244; Fassi, Farida/0000-0002-6423-7213; la rotonda, laura/0000-0002-6780-5829; Osculati, Bianca Maria/0000-0002-7246-060X; Amorim, Antonio/0000-0003-0638-2321; Coccaro, Andrea/0000-0003-2368-4559; Monzani, Simone/0000-0002-0479-2207; Grancagnolo, Francesco/0000-0002-9367-3380; Korol, Aleksandr/0000-0001-8448-218X; Karyukhin, Andrey/0000-0001-9087-4315; Smestad, Lillian/0000-0002-0244-8736; Giordani, Mario/0000-0002-0792-6039; Capua, Marcella/0000-0002-2443-6525; Di Micco, Biagio/0000-0002-4067-1592; Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; Doria, Alessandra/0000-0002-5381-2649; Vykydal, Zdenek/0000-0003-2329-0672; Olshevskiy, Alexander/0000-0002-8902-1793; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; KHODINOV, ALEKSANDR/0000-0003-3551-5808; O'Shea, Val/0000-0001-7183-1205; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Andreazza, Attilio/0000-0001-5161-5759; Carvalho, Joao/0000-0002-3015-7821; Mashinistov, Ruslan/0000-0001-7925-4676; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Hansen, John/0000-0002-8422-5543; Grancagnolo, Sergio/0000-0001-8490-8304; spagnolo, stefania/0000-0001-7482-6348; Ciubancan, Liviu Mihai/0000-0003-1837-2841; Camarri, Paolo/0000-0002-5732-5645; Tikhomirov, Vladimir/0000-0002-9634-0581; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; Ventura, Andrea/0000-0002-3368-3413; De, Kaushik/0000-0002-5647-4489; Mitsou, Vasiliki/0000-0002-1533-8886; White, Ryan/0000-0003-3589-5900; Joergensen, Morten/0000-0002-6790-9361; Riu, Imma/0000-0002-3742-4582; Mir, Lluisa-Maria/0000-0002-4276-715X; Della Pietra, Massimo/0000-0003-4446-3368; Petrucci, Fabrizio/0000-0002-5278-2206; Negrini, Matteo/0000-0003-0101-6963; Ferrer, Antonio/0000-0003-0532-711X FU CERN FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. NR 64 TC 16 Z9 16 U1 6 U2 150 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD OCT 21 PY 2013 IS 10 AR 130 DI 10.1007/JHEP10(2013)130 PG 50 WC Physics, Particles & Fields SC Physics GA 239SE UT WOS:000326044900001 ER PT J AU Chance, WM Bugaris, DE Sefat, AS zur Loye, HC AF Chance, W. Michael Bugaris, Daniel E. Sefat, Athena S. zur Loye, Hans-Conrad TI Crystal Growth of New Hexahydroxometallates Using a Hydroflux SO INORGANIC CHEMISTRY LA English DT Article ID NEUTRON POWDER DIFFRACTION; METAL-HYDROXIDES; AMPHOTERIC BEHAVIOR; MATERIALS DISCOVERY; MAGNETIC-PROPERTIES; TERNARY HYDROXIDES; OXIDES; SYSTEM; HYDROGARNETS; COMPOUND AB A series of seven compounds, Sr2Mn(OH)(6), Ba2Mn(OH)(6), Sr2Co(OH)(6), Ba2Co(OH)(6), Sr2Ni(OH)(6), Ba2Ni(OH)(6), and Ba2Cu(OH)(6), were synthesized using a low-melting hydroflux, a hybrid approach between aqueous hydrothermal and molten hydroxide flux techniques. Crystals of the hexahydroxometallates were obtained by dissolving appropriate amounts of alkaline-earth nitrates or hydroxides and transition-metal oxides, acetates, or chlorides in the hydroflux and reacting at 180-230 degrees C. The isostructural compounds all crystallize in the monoclinic space group P2(1)/n. The monoclinic structure consists of isolated transition-metal octahedra within a three-dimensional framework of corner- and edge-shared eight-coordinate, alkaline-earth polyhedra. Magnetic susceptibility data show that all compounds are simple paramagnets. Thermogravimetric analysis indicates that these hydroxides lose water between 215 and 350 degrees C and transform into oxide products, the identity of which depends on the metal cations present in the parent hexahydroxometallates. C1 [Chance, W. Michael; Bugaris, Daniel E.; zur Loye, Hans-Conrad] Univ S Carolina, Dept Chem & Biochem, Columbia, SC 29208 USA. [Sefat, Athena S.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP zur Loye, HC (reprint author), Univ S Carolina, Dept Chem & Biochem, Columbia, SC 29208 USA. EM zurloye@mailbox.sc.edu RI Sefat, Athena/R-5457-2016; OI Sefat, Athena/0000-0002-5596-3504; zur Loye, Hans-Conrad/0000-0001-7351-9098 FU NASA-EPSCoR program [520880]; U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division; USC selection committee FX The authors gratefully acknowledge financial support from the NASA-EPSCoR program through Award 520880. The research at ORNL was supported by the U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. Mary Anne Fitzpatrick, Dean, and the USC selection committee are gratefully acknowledged for supporting Michael Chance via a College of Arts and Sciences Dean's Dissertation Fellowship. NR 66 TC 11 Z9 11 U1 3 U2 21 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD OCT 21 PY 2013 VL 52 IS 20 BP 11723 EP 11733 DI 10.1021/ic400910g PG 11 WC Chemistry, Inorganic & Nuclear SC Chemistry GA 239ZX UT WOS:000326065600009 PM 24107084 ER PT J AU Wibowo, AC Malliakas, CD Chung, DY Im, J Freeman, AJ Kanatzidis, MG AF Wibowo, Arief C. Malliakas, Christos D. Chung, Duck Young Im, Jino Freeman, Arthur J. Kanatzidis, Mercouri G. TI Thallium Mercury Chalcobromides, TlHg(6)Q(4)Br(5) (Q = S, Se) SO INORGANIC CHEMISTRY LA English DT Article ID UP-CONVERSION LUMINESCENCE; SOLID-STATE; DIMENSIONAL REDUCTION; OPTICAL-PROPERTIES; CRYSTAL-STRUCTURE; CHALCOGENIDE HALIDES; IONIC LIQUIDS; = K; CHEMISTRY; CLUSTERS AB The new compounds TlHg(6)Q(4)Br(5) (Q = S, Se) are reported along with their syntheses, crystal structures, and thermal and optical properties, as well as electronic band structure calculations. Both compounds crystallize in the tetragonal I4/m space group with a = 14.145(1) angstrom, c = 8.803(1) angstrom, and d(calc) = 7.299 g/cm(3) for TlHg6S4Br5 (compound 1) and a = 14.518(2) angstrom, c = 8.782(1) angstrom, and d(calc) = 7.619 g/cm(3) for TlHg6Se4Br5 (compound 2). They consist of cuboid Hg(12)Q(3) building units interconnected by trigonal pyramids of BrHg3, forming a three-dimensional structure. The interstitial spaces are filled with thallium and bromide ions. Compounds 1 and 2 melt incongruently and show band gaps of 3.03 and 2.80 eV, respectively, which agree well with the calculated ones. First-principles electronic structure calculations at the density functional theory level reveal that both compounds have indirect band gaps, but there also exist direct transitions at energies similar to the indirect gaps. C1 [Wibowo, Arief C.; Malliakas, Christos D.; Chung, Duck Young; Kanatzidis, Mercouri G.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Malliakas, Christos D.; Kanatzidis, Mercouri G.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Im, Jino; Freeman, Arthur J.] Northwestern Univ, Dept Phys & Astron, Evanston, IL 60208 USA. RP Kanatzidis, MG (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM m-kanatzidis@northwestern.edu RI Wibowo, Arief/D-9418-2014 OI Wibowo, Arief/0000-0002-2454-4307 FU Office of Nonproliferation and Verification Research and Development under National Nuclear Security Administration of the U.S. Department of Energy [DE-AC02-06CH11357] FX This work was supported by the Office of Nonproliferation and Verification Research and Development under National Nuclear Security Administration of the U.S. Department of Energy under Contract No. DE-AC02-06CH11357. NR 53 TC 9 Z9 10 U1 0 U2 37 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD OCT 21 PY 2013 VL 52 IS 20 BP 11875 EP 11880 DI 10.1021/ic4014174 PG 6 WC Chemistry, Inorganic & Nuclear SC Chemistry GA 239ZX UT WOS:000326065600025 PM 24106977 ER PT J AU Jasper, AW Dawes, R AF Jasper, Ahren W. Dawes, Richard TI Non-Born-Oppenheimer molecular dynamics of the spin-forbidden reaction O(P-3)+CO(X-1 Sigma(+)) -> CO2((X)over-tilde(1)Sigma(+)(g)) SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID THERMAL UNIMOLECULAR REACTIONS; SURFACE HOPPING CALCULATIONS; TRANSITION-STATE THEORY; SELF-CONSISTENT-FIELD; ORBIT MATRIX-ELEMENTS; ELECTRONIC-TRANSITIONS; AB-INITIO; CO2 PHOTODISSOCIATION; COLLISION PROCESSES; CHEMICAL-REACTIONS AB The lowest-energy singlet (1 (1)A') and two lowest-energy triplet (1 (3)A' and 1 (3)A '') electronic states of CO2 are characterized using dynamically weighted multireference configuration interaction (dw-MRCI+Q) electronic structure theory calculations extrapolated to the complete basis set (CBS) limit. Global analytic representations of the dw-MRCI+Q/CBS singlet and triplet surfaces and of their CASSCF/aug-cc-pVQZ spin-orbit coupling surfaces are obtained via the interpolated moving least squares (IMLS) semiautomated surface fitting method. The spin-forbidden kinetics of the title reaction is calculated using the coupled IMLS surfaces and coherent switches with decay of mixing non-Born-Oppenheimer molecular dynamics. The calculated spin-forbidden association rate coefficient (corresponding to the high pressure limit of the rate coefficient) is 7-35 times larger at 1000-5000 K than the rate coefficient used in many detailed chemical models of combustion. A dynamical analysis of the multistate trajectories is presented. The trajectory calculations reveal direct (nonstatistical) and indirect (statistical) spin-forbidden reaction mechanisms and may be used to test the suitability of transition-state-theory-like statistical methods for spin-forbidden kinetics. Specifically, we consider the appropriateness of the "double passage" approximation, of assuming statistical distributions of seam crossings, and of applications of the unified statistical model for spin-forbidden reactions. (C) 2013 AIP Publishing LLC. C1 [Jasper, Ahren W.] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA. [Dawes, Richard] Missouri Univ Sci & Technol, Dept Chem, Rolla, MO 65409 USA. RP Jasper, AW (reprint author), Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA. EM ajasper@sandia.gov; dawesr@mst.edu RI Dawes, Richard/C-6344-2015; Jasper, Ahren/A-5292-2011 FU Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy. Sandia is a multiprogram laboratory operated by Sandia Corporation; Lockheed Martin Company; United States Department of Energy [DE-AC04-94-AL85000]; Office of Basic Energy Sciences, Division of Chemical Sciences, U.S. Department of Energy [DE-SC0010616] FX We thank Leonid Sheps and John Keifer for helpful conversations regarding the experimental kinetics literature. A.W.J. is supported by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy under Contract No. DE-AC04-94-AL85000. R.D. is supported by the Office of Basic Energy Sciences, Division of Chemical Sciences, U.S. Department of Energy under Contract No. DE-SC0010616. NR 85 TC 12 Z9 12 U1 3 U2 28 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD OCT 21 PY 2013 VL 139 IS 15 AR 154313 DI 10.1063/1.4825204 PG 13 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 240SF UT WOS:000326116600031 PM 24160519 ER PT J AU Perry, JW Dawes, R Wagner, AF Thompson, DL AF Perry, Jamin W. Dawes, Richard Wagner, Albert F. Thompson, Donald L. TI A classical trajectory study of the intramolecular dynamics, isomerization, and unimolecular dissociation of HO2 (vol 139, 084319, 2013) SO JOURNAL OF CHEMICAL PHYSICS LA English DT Correction C1 [Perry, Jamin W.; Thompson, Donald L.] Univ Missouri, Dept Chem, Columbia, MO 65211 USA. [Dawes, Richard] Missouri Univ Sci & Technol, Dept Chem, Rolla, MO 65409 USA. [Wagner, Albert F.] Argonne Natl Lab, Div Chem, Argonne, IL 60439 USA. RP Perry, JW (reprint author), Univ Missouri, Dept Chem, Columbia, MO 65211 USA. RI Dawes, Richard/C-6344-2015 NR 1 TC 0 Z9 0 U1 0 U2 7 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD OCT 21 PY 2013 VL 139 IS 15 AR 159903 DI 10.1063/1.4826557 PG 1 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 240SF UT WOS:000326116600061 ER PT J AU Lee, S Roseker, W Gutt, C Fischer, B Conrad, H Lehmkuhler, F Steinke, I Zhu, D Lemke, H Cammarata, M Fritz, DM Wochner, P Castro-Colin, M Hruszkewycz, SO Fuoss, PH Stephenson, GB Grubel, G Robert, A AF Lee, Sooheyong Roseker, W. Gutt, C. Fischer, B. Conrad, H. Lehmkuehler, F. Steinke, I. Zhu, D. Lemke, H. Cammarata, M. Fritz, D. M. Wochner, P. Castro-Colin, M. Hruszkewycz, S. O. Fuoss, P. H. Stephenson, G. B. Gruebel, G. Robert, A. TI Single shot speckle and coherence analysis of the hard X-ray free electron laser LCLS SO OPTICS EXPRESS LA English DT Article ID AMPLIFIED SPONTANEOUS-EMISSION; EXTREME-ULTRAVIOLET; WATER WINDOW; GAIN; RADIATION; SPECTROSCOPY; DIFFRACTION; OPERATION; REGION; NOISE AB The single shot based coherence properties of hard x-ray pulses from the Linac Coherent Light Source (LCLS) were measured by analyzing coherent diffraction patterns from nano-particles and gold nanopowder. The intensity histogram of the small angle x-ray scattering ring from nano-particles reveals the fully transversely coherent nature of the LCLS beam with a number of transverse mode < M-s > = 1.1. On the other hand, the speckle contrasts measured at a large wavevector yields information about the longitudinal coherence of the LCLS radiation after a silicon (111) monochromator. The quantitative agreement between our data and the simulation confirms a mean coherence time of 2.2 fs and a x-ray pulse duration of 29 fs. Finally the observed reduction of the speckle contrast generated by x-rays with pulse duration longer than 30 fs indicates ultrafast dynamics taking place at an atomic length scale prior to the permanent sample damage. (C) 2013 Optical Society of America C1 [Lee, Sooheyong] KRISS, Taejon 305600, South Korea. [Lee, Sooheyong; Roseker, W.; Gutt, C.; Fischer, B.; Conrad, H.; Lehmkuehler, F.; Steinke, I.; Gruebel, G.] DESY, HASYLAB, D-22607 Hamburg, Germany. [Zhu, D.; Lemke, H.; Cammarata, M.; Fritz, D. M.; Robert, A.] SLAC Natl Accelerator Lab, Linac Coherent Light Source, Menlo Pk, CA 94025 USA. [Wochner, P.; Castro-Colin, M.] Max Planck Inst Intelligente Syst, D-70569 Stuttgart, Germany. [Hruszkewycz, S. O.; Fuoss, P. H.; Stephenson, G. B.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Lee, S (reprint author), KRISS, Taejon 305600, South Korea. EM sooheyong@gmail.com RI Cammarata, Marco/C-2322-2008; Lemke, Henrik Till/N-7419-2016; Lehmkuhler, Felix/C-2367-2017; OI Cammarata, Marco/0000-0003-3013-1186; Lemke, Henrik Till/0000-0003-1577-8643; Lehmkuhler, Felix/0000-0003-1289-995X; Conrad, Heiko/0000-0002-1014-9605 FU U.S. Department of Energy's Office of Basic Energy Sciences; DoE; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; Converging Research Center Program through the Ministry of Science, ICT and Future Planning, Korea [2013K000307]; Deutsche Forschungsgemeinschaft FX The Linac Coherent Light Source is funded by the U.S. Department of Energy's Office of Basic Energy Sciences and led by the SLAC National Accelerator Laboratory, which is operated by Stanford University for the DoE. P. H. F. and G. B. S. were supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. This research was supported by the Converging Research Center Program through the Ministry of Science, ICT and Future Planning, Korea (2013K000307). The Au nanopowder samples were supplied by A. Plech. P. W., M. C.-C. We thank Y. Ding and Z. Huang for helpful discussions. The authors acknowledge financial support by the Deutsche Forschungsgemeinschaft within the framework of the graduate school 1355 Physics with new advanced coherent radiation sources. NR 41 TC 10 Z9 10 U1 0 U2 27 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD OCT 21 PY 2013 VL 21 IS 21 BP 24647 EP 24664 DI 10.1364/OE.21.024647 PG 18 WC Optics SC Optics GA 240HI UT WOS:000326085600023 PM 24150309 ER PT J AU Guzman-Verri, GG Littlewood, PB Varma, CM AF Guzman-Verri, G. G. Littlewood, P. B. Varma, C. M. TI Paraelectric and ferroelectric states in a model for relaxor ferroelectrics SO PHYSICAL REVIEW B LA English DT Article ID GLASSY POLARIZATION BEHAVIOR; FIELD ISING-MODEL; SINGLE-CRYSTALS; PHASE-TRANSITION; LEAD TITANATE; X-RAY; PBMG1/3NB2/3O3; CERAMICS; ORDER; PEROVSKITES AB We study the free-energy landscape of a minimal model for relaxor ferroelectrics. Using a variational method which includes leading correlations beyond the mean-field approximation as well as disorder averaging at the level of a simple replica theory, we find metastable paraelectric states with a stability region that extends to zero temperature. The free energy of such states exhibits an essential singularity for weak compositional disorder pointing to their necessary occurrence. Ferroelectric states appear as local minima in the free energy at high temperatures and become stable below a coexistence temperature T-c. We calculate the phase diagram in the electric-field-temperature plane and find a coexistence line of the polar and nonpolar phases which ends at a critical point. First-order phase transitions are induced for fields sufficiently large to cross the region of stability of the metastable paraelectric phase. These polar and nonpolar states have distinct structure factors from those of conventional ferroelectrics. We use this theoretical framework to compare and gain physical understanding of various experimental results in typical relaxors. C1 [Guzman-Verri, G. G.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Littlewood, P. B.] Argonne Natl Lab, Argonne, IL 60439 USA. [Littlewood, P. B.] Univ Chicago, James Franck Inst, Chicago, IL 60637 USA. [Varma, C. M.] Univ Calif Riverside, Dept Phys & Astron, Riverside, CA 92521 USA. RP Guzman-Verri, GG (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. RI Guzman-Verri, G/H-6031-2011 FU US Department of Energy, Office of Basic Energy Sciences [DE-AC02-06CH11357]; UC Lab Fee Program [09-LR-01-118286-HELF] FX GGGV and PBL acknowledge useful discussions with Stephen Streiffer and Ray Osborn. Work at Argonne National Laboratory is supported by the US Department of Energy, Office of Basic Energy Sciences under Contract No. DE-AC02-06CH11357. Work at University of California (UC) Riverside is supported by the UC Lab Fee Program No. 09-LR-01-118286-HELF. GGGV and CMV wish to thank other principal investigators with whom the UC grant was issued: Frances Hellman, Albert Migliori, and Alexandra Navrotsky. NR 82 TC 13 Z9 13 U1 3 U2 33 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 21 PY 2013 VL 88 IS 13 AR 134106 DI 10.1103/PhysRevB.88.134106 PG 9 WC Physics, Condensed Matter SC Physics GA 240HL UT WOS:000326085900001 ER PT J AU McElroy, CA Hamlin, JJ White, BD McGuire, MA Sales, BC Maple, MB AF McElroy, C. A. Hamlin, J. J. White, B. D. McGuire, M. A. Sales, B. C. Maple, M. B. TI Magnetotransport properties of single-crystalline LaFeAsO SO PHYSICAL REVIEW B LA English DT Article ID SUPERCONDUCTIVITY; METAL AB Measurements of magnetization, specific heat, electrical resistivity, Hall effect, and magnetoresistance on single crystalline samples of LaFeAsO grown in a NaAs flux are reported. While this material is known to be a semimetal, the temperature dependence of the electrical resistivity data presented herein is reminiscent of semiconducting behavior and exhibits distinct features associated with a structural transition and spin density wave (SDW) order. Low-temperature x-ray diffraction measurements have confirmed that the structural transition in these samples occurs near 140 K, compared to a transition temperature of 156 K observed in polycrystalline samples. Magnetoresistance and Hall coefficient measurements were performed in magnetic fields up to 9 T applied perpendicular to the basal plane using a van der Pauw configuration. The charge carrier density and mobility indicate that electrons are the majority charge carriers and exhibit features indicative of the structural transition and SDW formation. Isotherms of magnetoresistivity measured as a function of magnetic field can be scaled onto a single curve. C1 [McElroy, C. A.; Hamlin, J. J.; White, B. D.; Maple, M. B.] Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. [McElroy, C. A.; Hamlin, J. J.; White, B. D.; Maple, M. B.] Univ Calif San Diego, Ctr Adv Nanosci, La Jolla, CA 92093 USA. [McGuire, M. A.; Sales, B. C.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Maple, MB (reprint author), Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. EM mbmaple@ucsd.edu RI McGuire, Michael/B-5453-2009 OI McGuire, Michael/0000-0003-1762-9406 FU US AFOSR-MURI [FA9550-09-1-0603]; US DOE [DE-FG02-04-ER46105]; US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division FX Sample synthesis was funded by the US AFOSR-MURI (Grant FA9550-09-1-0603). Physical properties measurements were supported by the US DOE (Grant DE-FG02-04-ER46105). Research at Oak Ridge (MAM and BCS) was supported by the US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. NR 29 TC 3 Z9 3 U1 1 U2 33 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 21 PY 2013 VL 88 IS 13 AR 134513 DI 10.1103/PhysRevB.88.134513 PG 7 WC Physics, Condensed Matter SC Physics GA 240HL UT WOS:000326085900006 ER PT J AU Wen, JS Li, SC Xu, ZJ Zhang, C Matsuda, M Sobolev, O Park, JT Christianson, AD Bourret-Courchesne, E Li, Q Gu, GD Lee, DH Tranquada, JM Xu, GY Birgeneau, RJ AF Wen, Jinsheng Li, Shichao Xu, Zhijun Zhang, Cheng Matsuda, M. Sobolev, O. Park, J. T. Christianson, A. D. Bourret-Courchesne, E. Li, Qiang Gu, Genda Lee, Dung-Hai Tranquada, J. M. Xu, Guangyong Birgeneau, R. J. TI Enhanced low-energy magnetic excitations via suppression of the itinerancy in Fe0.98-zCuzTe0.5Se0.5 SO PHYSICAL REVIEW B LA English DT Article ID SUPERCONDUCTORS AB We have performed resistivity and inelastic neutron scattering measurements on three samples of Fe0.98-zCuzTe0.5Se0.5 with z = 0, 0.02, and 0.1. It is found that with increasing Cu doping the sample's resistivity deviates progressively from that of a metal. However, in contrast to expectations that replacing Fe with Cu would suppress the magnetic correlations, the low-energy (<= 12 meV) magnetic scattering is enhanced in strength, with greater spectral weight and longer dynamical spin-spin correlation lengths. Such enhancements can be a consequence of either enlarged local moments or a slowing down of the spin fluctuations. In either case, the localization of the conduction states induced by the Cu doping should play a critical role. Our results are not applicable to models that treat 3d transition metal dopants simply as effective electron donors. C1 [Wen, Jinsheng; Li, Shichao] Nanjing Univ, Natl Lab Solid State Microstruct, Ctr Superconducting Phys & Mat, Nanjing 210093, Jiangsu, Peoples R China. [Wen, Jinsheng; Li, Shichao] Nanjing Univ, Dept Phys, Nanjing 210093, Jiangsu, Peoples R China. [Wen, Jinsheng; Lee, Dung-Hai; Birgeneau, R. J.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Wen, Jinsheng; Lee, Dung-Hai; Birgeneau, R. J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Xu, Zhijun; Zhang, Cheng; Li, Qiang; Gu, Genda; Tranquada, J. M.; Xu, Guangyong] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Matsuda, M.; Christianson, A. D.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Sobolev, O.; Park, J. T.] Tech Univ Munich, Forsch Neutronenquelle Heinz Maier Leibnitz FRM 2, D-85747 Garching, Germany. [Bourret-Courchesne, E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Life Sci Div, Berkeley, CA 94720 USA. [Birgeneau, R. J.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. RP Wen, JS (reprint author), Nanjing Univ, Natl Lab Solid State Microstruct, Ctr Superconducting Phys & Mat, Nanjing 210093, Jiangsu, Peoples R China. EM jwen@nju.edu.cn RI Wen, Jinsheng/F-4209-2010; xu, zhijun/A-3264-2013; Tranquada, John/A-9832-2009; christianson, andrew/A-3277-2016; Matsuda, Masaaki/A-6902-2016; Park, Jitae/G-1358-2016; Xu, Guangyong/A-8707-2010; Sobolev, Oleg/P-5983-2016; Zhang, Cheng/R-6593-2016 OI Wen, Jinsheng/0000-0001-5864-1466; xu, zhijun/0000-0001-7486-2015; Tranquada, John/0000-0003-4984-8857; christianson, andrew/0000-0003-3369-5884; Matsuda, Masaaki/0000-0003-2209-9526; Park, Jitae/0000-0001-6565-0192; Xu, Guangyong/0000-0003-1441-8275; Zhang, Cheng/0000-0001-6531-4703 FU Office of Basic Energy Sciences, Division of Materials Science and Engineering, US Department of Energy [DE-AC02-05CH11231, DE-AC02-98CH10886]; Division of Scientific User Facilities FX We are grateful for the stimulating discussions with Wei Ku, Weiguo Yin, Tom Berlijn, Qianghua Wang, Jianxin Li, and Haihu Wen. The work at Lawrence Berkeley National Laboratory and Brookhaven National Laboratory was supported by the Office of Basic Energy Sciences, Division of Materials Science and Engineering, US Department of Energy, under Contracts No. DE-AC02-05CH11231 and No. DE-AC02-98CH10886, respectively. Research at Oak Ridge National Laboratory's High Flux Isotope Reactor was sponsored by the Division of Scientific User Facilities of the same office. NR 37 TC 11 Z9 11 U1 3 U2 18 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 21 PY 2013 VL 88 IS 14 AR 144509 DI 10.1103/PhysRevB.88.144509 PG 5 WC Physics, Condensed Matter SC Physics GA 240HS UT WOS:000326086700007 ER PT J AU Hartley, DJ Pedicini, EE Janssens, RVF Riedinger, LL Riley, MA Wang, X Miller, S Ayangeakaa, AD Carpenter, MP Carroll, JJ Cavey, J Chiara, CJ Chowdhury, P Garg, U Hota, SS Jackson, EG Kondev, FG Lauritsen, T Litz, M Ma, WC Matta, J Paul, ES Simpson, J Vanhoy, JR Zhu, S AF Hartley, D. J. Pedicini, E. E. Janssens, R. V. F. Riedinger, L. L. Riley, M. A. Wang, X. Miller, S. Ayangeakaa, A. D. Carpenter, M. P. Carroll, J. J. Cavey, J. Chiara, C. J. Chowdhury, P. Garg, U. Hota, S. S. Jackson, E. G. Kondev, F. G. Lauritsen, T. Litz, M. Ma, W. C. Matta, J. Paul, E. S. Simpson, J. Vanhoy, J. R. Zhu, S. TI Possible deformation evolution in the pi i(13/2) structure of Re-171 SO PHYSICAL REVIEW C LA English DT Article ID NUCLEAR-DATA SHEETS; COINCIDENCE DATA; WOBBLING MODE; CONFIGURATION; EXCITATIONS; LU-167; PHONON; BAND AB The phenomenon of wobbling can only occur for a nuclear shape with stable triaxial deformation. To date, only a few examples of this exotic collective mode have been observed in lutetium and tantalum isotopes. A search for a wobbling sequence was performed in Re-171 to determine if this feature can be observed in Z > 73 nuclei. No evidence was found for wobbling; however, an interaction between the pi i(13/2) sequence and another positive-parity band may give an indication on why wobbling may not occur in this nucleus. The level scheme for Re-171 was significantly extended and interpretations for the decay sequences are proposed within the context of the cranked shell model. C1 [Hartley, D. J.; Pedicini, E. E.; Cavey, J.; Vanhoy, J. R.] US Naval Acad, Dept Phys, Annapolis, MD 21402 USA. [Janssens, R. V. F.; Carpenter, M. P.; Chiara, C. J.; Lauritsen, T.; Zhu, S.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Riedinger, L. L.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Riley, M. A.; Wang, X.; Miller, S.] Florida State Univ, Dept Phys, Tallahassee, FL 32306 USA. [Ayangeakaa, A. D.; Garg, U.; Matta, J.] Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. [Carroll, J. J.; Litz, M.] Army Res Lab, Adelphi, MD 20783 USA. [Chiara, C. J.] Univ Maryland, Dept Chem & Biochem, College Pk, MD 20742 USA. [Chiara, C. J.; Kondev, F. G.] Argonne Natl Lab, Nucl Engn Div, Argonne, IL 60439 USA. [Chowdhury, P.; Hota, S. S.; Jackson, E. G.] Univ Massachusetts, Dept Phys, Lowell, MA 01854 USA. [Ma, W. C.] Mississippi State Univ, Dept Phys, Mississippi State, MS 39762 USA. [Paul, E. S.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 7ZE, Merseyside, England. [Simpson, J.] STFC Daresbury Lab, Warrington WA4 4AD, Cheshire, England. RP Hartley, DJ (reprint author), US Naval Acad, Dept Phys, Annapolis, MD 21402 USA. RI Carpenter, Michael/E-4287-2015; Ayangeakaa, Akaa/F-3683-2015 OI Carpenter, Michael/0000-0002-3237-5734; Ayangeakaa, Akaa/0000-0003-1679-3175 FU National Science Foundation [PHY-1203100, PHY-0754674, PHY-1068192]; U.S. Department of Energy, Office of Nuclear Physics [DE-AC02-06CH11357, DE-FG02-94ER40848, DE-FG02-96ER40983, DE-FG02-94ER40834, DE-FG02-95ER40939]; United Kingdom Science and Technology Facilities Council FX The authors thank the ANL operations staff at Gammasphere and gratefully acknowledge the efforts of J. P. Greene for target preparation. We thank D. C. Radford and H. Q. Jin for their software support. This work was funded by the National Science Foundation under Grants No. PHY-1203100 (USNA), No. PHY-0754674 (FSU), and No. PHY-1068192 (ND), the U.S. Department of Energy, Office of Nuclear Physics, under Contracts No. DE-AC02-06CH11357 (ANL), No. DE-FG02-94ER40848 (UML), No. DE-FG02-96ER40983 (UT), No. DE-FG02-94ER40834 (UMCP), and No. DE-FG02-95ER40939 (MSU), as well as the United Kingdom Science and Technology Facilities Council. NR 36 TC 1 Z9 1 U1 0 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD OCT 21 PY 2013 VL 88 IS 4 AR 044323 DI 10.1103/PhysRevC.88.044323 PG 15 WC Physics, Nuclear SC Physics GA 240KY UT WOS:000326096000003 ER PT J AU Abazov, VM Abbott, B Acharya, BS Adams, M Adams, T Agnew, JP Alexeev, GD Alkhazov, G Alton, A Askew, A Atkins, S Augsten, K Avila, C Badaud, F Bagby, L Baldin, B Bandurin, DV Banerjee, S Barberis, E Baringer, P Bartlett, JF Bassler, U Bazterra, V Bean, A Begalli, M Bellantoni, L Beri, SB Bernardi, G Bernhard, R Bertram, I Besancon, M Beuselinck, R Bhat, PC Bhatia, S Bhatnagar, V Blazey, G Blessing, S Bloom, K Boehnlein, A Boline, D Boos, EE Borissov, G Brandt, A Brandt, O Brock, R Bross, A Brown, D Bu, XB Buehler, M Buescher, V Bunichev, V Burdin, S Buszello, CP Camacho-Perez, E Casey, BCK Castilla-Valdez, H Caughron, S Chakrabarti, S Chan, KM Chandra, A Chapon, E Chen, G Cho, SW Choi, S Choudhary, B Cihangir, S Claes, D Clutter, J Cooke, M Cooper, WE Corcoran, M Couderc, F Cousinou, MC Cutts, D Das, A Davies, G de Jong, SJ De La Cruz-Burelo, E Deliot, F Demina, R Denisov, D Denisov, SP Desai, S Deterre, C DeVaughan, K Diehl, HT Diesburg, M Ding, PF Dominguez, A Dubey, A Dudko, LV Duperrin, A Dutt, S Eads, M Edmunds, D Ellison, J Elvira, VD Enari, Y Evans, H Evdokimov, VN Feng, L Ferbel, T Fiedler, F Filthaut, F Fisher, W Fisk, HE Fortner, M Fox, H Fuess, S Garcia-Bellido, A Garcia-Gonzalez, JA Gavrilov, V Geng, W Gerber, CE Gershtein, Y Ginther, G Golovanov, G Grannis, PD Greder, S Greenlee, H Grenier, G Gris, P Grivaz, JF Grohsjean, A Grunendahl, S Grunewald, MW Guillemin, T Gutierrez, G Gutierrez, P Haley, J Han, L Harder, K Harel, A Hauptman, JM Hays, J Head, T Hebbeker, T Hedin, D Hegab, H Heinson, AP Heintz, U Hensel, C Cruz, IHD Herner, K Hesketh, G Hildreth, MD Hirosky, R Hoang, T Hobbs, JD Hoeneisen, B Hogan, J Hohlfeld, M Holzbauer, JL Howley, I Hubacek, Z Hynek, V Iashvili, I Ilchenko, Y Illingworth, R Ito, AS Jabeen, S Jaffre, M Jayasinghe, A Jeong, MS Jesik, R Jiang, P Johns, K Johnson, E Johnson, M Jonckheere, A Jonsson, P Joshi, J Jung, AW Juste, A Kajfasz, E Karmanov, D Katsanos, I Kehoe, R Kermiche, S Khalatyan, N Khanov, A Kharchilava, A Kharzheev, YN Kiselevich, I Kohli, JM Kozelov, AV Kraus, J Kumar, A Kupco, A Kurca, T Kuzmin, VA Lammers, S Lebrun, P Lee, HS Lee, SW Lee, WM Lei, X Lellouch, J Li, D Li, H Li, L Li, QZ Lim, JK Lincoln, D Linnemann, J Lipaev, VV Lipton, R Liu, H Liu, Y Lobodenko, A Lokajicek, M de Sa, RL Luna-Garcia, R Lyon, AL Maciel, AKA Madar, R Magana-Villalba, R Malik, S Malyshev, VL Mansour, J Martinez-Ortega, J McCarthy, R McGivern, CL Meijer, MM Melnitchouk, A Menezes, D Mercadante, PG Merkin, M Meyer, A Meyer, J Miconi, F Mondal, NK Mulhearn, M Nagy, E Narain, M Nayyar, R Neal, HA Negret, JP Neustroev, P Nguyen, HT Nunnemann, T Orduna, J Osman, N Osta, J Pal, A Parashar, N Parihar, V Park, SK Partridge, R Parua, N Patwa, A Penning, B Perfilov, M Peters, Y Petridis, K Petrillo, G Petroff, P Pleier, MA Podstavkov, VM Popov, AV Prewitt, M Price, D Prokopenko, N Qian, J Quadt, A Quinn, B Ratoff, PN Razumov, I Ripp-Baudot, I Rizatdinova, F Rominsky, M Ross, A Royon, C Rubinov, P Ruchti, R Sajot, G Sanchez-Hernandez, A Sanders, MP Santos, AS Savage, G Sawyer, L Scanlon, T Schamberger, RD Scheglov, Y Schellman, H Schwanenberger, C Schwienhorst, R Sekaric, J Severini, H Shabalina, E Shary, V Shaw, S Shchukin, AA Simak, V Skachkov, NB Skubic, P Slattery, P Smirnov, D Snow, GR Snow, J Snyder, S Soldner-Rembold, S Sonnenschein, L Soustruznik, K Stark, J Stoyanova, DA Strauss, M Suter, L Svoisky, P Titov, M Tokmenin, VV Tsai, YT Tsybychev, D Tuchming, B Tully, C Uvarov, L Uvarov, S Uzunyan, S Van Kooten, R van Leeuwen, WM Varelas, N Varnes, EW Vasilyev, IA Verkheev, AY Vertogradov, LS Verzocchi, M Vesterinen, M Vilanova, D Vokac, P Wahl, HD Wang, MHLS Warchol, J Watts, G Wayne, M Weichert, J Welty-Rieger, L Williams, MRJ Wilson, GW Wobisch, M Wood, DR Wyatt, TR Xie, Y Yamada, R Yang, S Yasuda, T Yatsunenko, YA Ye, W Ye, Z Yin, H Yip, K Youn, SW Yu, JM Zennamo, J Zhao, TG Zhou, B Zhu, J Zielinski, M Zieminska, D Zivkovic, L AF Abazov, V. M. Abbott, B. Acharya, B. S. Adams, M. Adams, T. Agnew, J. P. Alexeev, G. D. Alkhazov, G. Alton, A. Askew, A. Atkins, S. Augsten, K. Avila, C. Badaud, F. Bagby, L. Baldin, B. Bandurin, D. V. Banerjee, S. Barberis, E. Baringer, P. Bartlett, J. F. Bassler, U. Bazterra, V. Bean, A. Begalli, M. Bellantoni, L. Beri, S. B. Bernardi, G. Bernhard, R. Bertram, I. Besancon, M. Beuselinck, R. Bhat, P. C. Bhatia, S. Bhatnagar, V. Blazey, G. Blessing, S. Bloom, K. Boehnlein, A. Boline, D. Boos, E. E. Borissov, G. Brandt, A. Brandt, O. Brock, R. Bross, A. Brown, D. Bu, X. B. Buehler, M. Buescher, V. Bunichev, V. Burdin, S. Buszello, C. P. Camacho-Perez, E. Casey, B. C. K. Castilla-Valdez, H. Caughron, S. Chakrabarti, S. Chan, K. M. Chandra, A. Chapon, E. Chen, G. Cho, S. W. Choi, S. Choudhary, B. Cihangir, S. Claes, D. Clutter, J. Cooke, M. Cooper, W. E. Corcoran, M. Couderc, F. Cousinou, M. -C. Cutts, D. Das, A. Davies, G. de Jong, S. J. De La Cruz-Burelo, E. Deliot, F. Demina, R. Denisov, D. Denisov, S. P. Desai, S. Deterre, C. DeVaughan, K. Diehl, H. T. Diesburg, M. Ding, P. F. Dominguez, A. Dubey, A. Dudko, L. V. Duperrin, A. Dutt, S. Eads, M. Edmunds, D. Ellison, J. Elvira, V. D. Enari, Y. Evans, H. Evdokimov, V. N. Feng, L. Ferbel, T. Fiedler, F. Filthaut, F. Fisher, W. Fisk, H. E. Fortner, M. Fox, H. Fuess, S. Garcia-Bellido, A. Garcia-Gonzalez, J. A. Gavrilov, V. Geng, W. Gerber, C. E. Gershtein, Y. Ginther, G. Golovanov, G. Grannis, P. D. Greder, S. Greenlee, H. Grenier, G. Gris, Ph. Grivaz, J. -F. Grohsjean, A. Gruenendahl, S. Gruenewald, M. W. Guillemin, T. Gutierrez, G. Gutierrez, P. Haley, J. Han, L. Harder, K. Harel, A. Hauptman, J. M. Hays, J. Head, T. Hebbeker, T. Hedin, D. Hegab, H. Heinson, A. P. Heintz, U. Hensel, C. Heredia-De La Cruz, I. Herner, K. Hesketh, G. Hildreth, M. D. Hirosky, R. Hoang, T. Hobbs, J. D. Hoeneisen, B. Hogan, J. Hohlfeld, M. Holzbauer, J. L. Howley, I. Hubacek, Z. Hynek, V. Iashvili, I. Ilchenko, Y. Illingworth, R. Ito, A. S. Jabeen, S. Jaffre, M. Jayasinghe, A. Jeong, M. S. Jesik, R. Jiang, P. Johns, K. Johnson, E. Johnson, M. Jonckheere, A. Jonsson, P. Joshi, J. Jung, A. W. Juste, A. Kajfasz, E. Karmanov, D. Katsanos, I. Kehoe, R. Kermiche, S. Khalatyan, N. Khanov, A. Kharchilava, A. Kharzheev, Y. N. Kiselevich, I. Kohli, J. M. Kozelov, A. V. Kraus, J. Kumar, A. Kupco, A. Kurca, T. Kuzmin, V. A. Lammers, S. Lebrun, P. Lee, H. S. Lee, S. W. Lee, W. M. Lei, X. Lellouch, J. Li, D. Li, H. Li, L. Li, Q. Z. Lim, J. K. Lincoln, D. Linnemann, J. Lipaev, V. V. Lipton, R. Liu, H. Liu, Y. Lobodenko, A. Lokajicek, M. de Sa, R. Lopes Luna-Garcia, R. Lyon, A. L. Maciel, A. K. A. Madar, R. Magana-Villalba, R. Malik, S. Malyshev, V. L. Mansour, J. Martinez-Ortega, J. McCarthy, R. McGivern, C. L. Meijer, M. M. Melnitchouk, A. Menezes, D. Mercadante, P. G. Merkin, M. Meyer, A. Meyer, J. Miconi, F. Mondal, N. K. Mulhearn, M. Nagy, E. Narain, M. Nayyar, R. Neal, H. A. Negret, J. P. Neustroev, P. Nguyen, H. T. Nunnemann, T. Orduna, J. Osman, N. Osta, J. Pal, A. Parashar, N. Parihar, V. Park, S. K. Partridge, R. Parua, N. Patwa, A. Penning, B. Perfilov, M. Peters, Y. Petridis, K. Petrillo, G. Petroff, P. Pleier, M. -A. Podstavkov, V. M. Popov, A. V. Prewitt, M. Price, D. Prokopenko, N. Qian, J. Quadt, A. Quinn, B. Ratoff, P. N. Razumov, I. Ripp-Baudot, I. Rizatdinova, F. Rominsky, M. Ross, A. Royon, C. Rubinov, P. Ruchti, R. Sajot, G. Sanchez-Hernandez, A. Sanders, M. P. Santos, A. S. Savage, G. Sawyer, L. Scanlon, T. Schamberger, R. D. Scheglov, Y. Schellman, H. Schwanenberger, C. Schwienhorst, R. Sekaric, J. Severini, H. Shabalina, E. Shary, V. Shaw, S. Shchukin, A. A. Simak, V. Skachkov, N. B. Skubic, P. Slattery, P. Smirnov, D. Snow, G. R. Snow, J. Snyder, S. Soeldner-Rembold, S. Sonnenschein, L. Soustruznik, K. Stark, J. Stoyanova, D. A. Strauss, M. Suter, L. Svoisky, P. Titov, M. Tokmenin, V. V. Tsai, Y. -T. Tsybychev, D. Tuchming, B. Tully, C. Uvarov, L. Uvarov, S. Uzunyan, S. Van Kooten, R. van Leeuwen, W. M. Varelas, N. Varnes, E. W. Vasilyev, I. A. Verkheev, A. Y. Vertogradov, L. S. Verzocchi, M. Vesterinen, M. Vilanova, D. Vokac, P. Wahl, H. D. Wang, M. H. L. S. Warchol, J. Watts, G. Wayne, M. Weichert, J. Welty-Rieger, L. Williams, M. R. J. Wilson, G. W. Wobisch, M. Wood, D. R. Wyatt, T. R. Xie, Y. Yamada, R. Yang, S. Yasuda, T. Yatsunenko, Y. A. Ye, W. Ye, Z. Yin, H. Yip, K. Youn, S. W. Yu, J. M. Zennamo, J. Zhao, T. G. Zhou, B. Zhu, J. Zielinski, M. Zieminska, D. Zivkovic, L. CA D0 Collaboration TI Measurement of the differential cross section of photon plus jet production in p(p)over-bar collisions at root s=1.96 TeV SO PHYSICAL REVIEW D LA English DT Article ID DEEP-INELASTIC SCATTERING; GLUON DISTRIBUTION; PARTON DISTRIBUTIONS; PP COLLISIONS; COLLIDER; HERA; LHC; PHOTOPRODUCTION; CONSTRAINTS; NUCLEON AB We study the process of associated photon and jet production, p (p) over bar -> gamma + jet + X, using 8.7 fb(-1) of integrated luminosity collected by the D0 detector at the Fermilab Tevatron Collider at a center-of-mass energy root s = 1.96 TeV. Photons are reconstructed with rapidity vertical bar y(gamma)vertical bar < 1.0 or 1.5 < vertical bar y(gamma)vertical bar < 2.5 and transverse momentum p(T)(gamma) > 20 GeV. The highest-p(T) jet is required to be in one of four rapidity regions up to vertical bar y(jet)vertical bar <= 3.2. For each rapidity configuration we measure the differential cross sections in p(T)(gamma) separately for events with the same sign (y(gamma)y(jet) > 0) and opposite signs (y(gamma)y(jet) <= 0) of photon and jet rapidities. We compare the measured triple-differential cross sections, d(3)sigma/dp(T)(gamma)dy(gamma)dy(jet), to next-to-leading order (NLO) perturbative QCD calculations using different sets of parton distribution functions, and to predictions from the SHERPA and PYTHIA Monte Carlo event generators. The NLO calculations are found to be in general agreement with the data but do not describe all kinematic regions. C1 [Maciel, A. K. A.; Santos, A. S.] Ctr Brasileiro Pesquisas Fis, LAFEX, Rio De Janeiro, Brazil. [Begalli, M.] Univ Estado Rio de Janeiro, BR-20550011 Rio De Janeiro, Brazil. [Mercadante, P. G.] Univ Fed ABC, Santo Andre, Brazil. [Han, L.; Jiang, P.; Liu, Y.; Yang, S.] Univ Sci & Technol China, Hefei 230026, Peoples R China. [Avila, C.; Negret, J. P.] Univ Los Andes, Bogota, Colombia. [Soustruznik, K.] Charles Univ Prague, Fac Math & Phys, Ctr Particle Phys, Prague, Czech Republic. [Augsten, K.; Hubacek, Z.; Hynek, V.; Simak, V.; Vokac, P.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Kupco, A.; Lokajicek, M.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Hoeneisen, B.] Univ San Francisco Quito, Quito, Ecuador. [Badaud, F.; Gris, Ph.] Univ Clermont Ferrand, LPC, CNRS, IN2P3, Clermont, France. [Sajot, G.; Stark, J.] Univ Grenoble 1, CNRS, LPSC, IN2P3,Inst Natl Polytech Grenoble, Grenoble, France. [Cousinou, M. -C.; Duperrin, A.; Geng, W.; Kajfasz, E.; Kermiche, S.; Nagy, E.; Osman, N.] Aix Marseille Univ, CPPM, CNRS, IN2P3, Marseille, France. [Grivaz, J. -F.; Guillemin, T.; Jaffre, M.; Petroff, P.] Univ Paris 11, CNRS, LAL, IN2P3, F-91405 Orsay, France. [Bernardi, G.; Brown, D.; Enari, Y.; Lellouch, J.; Li, D.; Zivkovic, L.] Univ Paris 06, LPNHE, Paris, France. [Bernardi, G.; Brown, D.; Enari, Y.; Lellouch, J.; Li, D.; Zivkovic, L.] Univ Paris 07, CNRS, IN2P3, Paris, France. [Bassler, U.; Besancon, M.; Chapon, E.; Couderc, F.; Deliot, F.; Grohsjean, A.; Hubacek, Z.; Royon, C.; Shary, V.; Titov, M.; Tuchming, B.; Vilanova, D.] CEA, Irfu, Saclay, France. [Greder, S.; Miconi, F.; Ripp-Baudot, I.] Univ Strasbourg, IPHC, CNRS, IN2P3, Strasbourg, France. [Grenier, G.; Kurca, T.; Lebrun, P.] Univ Lyon 1, CNRS, IPNL, IN2P3, F-69622 Villeurbanne, France. [Grenier, G.; Kurca, T.; Lebrun, P.] Univ Lyon, Lyon, France. [Hebbeker, T.; Meyer, A.; Sonnenschein, L.] Rhein Westfal TH Aachen, Phys Inst A3, Aachen, Germany. [Bernhard, R.; Madar, R.] Univ Freiburg, Inst Phys, D-79106 Freiburg, Germany. [Brandt, O.; Deterre, C.; Hensel, C.; Mansour, J.; Meyer, J.; Peters, Y.; Quadt, A.; Shabalina, E.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Buescher, V.; Fiedler, F.; Hohlfeld, M.; Weichert, J.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Nunnemann, T.; Sanders, M. P.] Univ Munich, Munich, Germany. [Beri, S. B.; Bhatnagar, V.; Dutt, S.; Kohli, J. M.] Panjab Univ, Chandigarh 160014, India. [Choudhary, B.; Dubey, A.] Univ Delhi, Delhi 110007, India. [Acharya, B. S.; Banerjee, S.; Mondal, N. K.] Tata Inst Fundamental Res, Bombay 400005, Maharashtra, India. [Gruenewald, M. W.] Univ Coll Dublin, Dublin 2, Ireland. [Cho, S. W.; Choi, S.; Jeong, M. S.; Lee, H. S.; Lim, J. K.; Park, S. K.] Korea Univ, Korea Detector Lab, Seoul, South Korea. [Camacho-Perez, E.; Castilla-Valdez, H.; De La Cruz-Burelo, E.; Garcia-Gonzalez, J. A.; Heredia-De La Cruz, I.; Luna-Garcia, R.; Magana-Villalba, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.] CINVESTAV, Mexico City 14000, DF, Mexico. [de Jong, S. J.; Filthaut, F.; Meijer, M. M.; van Leeuwen, W. M.] Nikhef, Amsterdam, Netherlands. [de Jong, S. J.; Filthaut, F.; Meijer, M. M.] Radboud Univ Nijmegen, NL-6525 ED Nijmegen, Netherlands. [Abazov, V. M.; Alexeev, G. D.; Golovanov, G.; Kharzheev, Y. N.; Malyshev, V. L.; Skachkov, N. B.; Tokmenin, V. V.; Verkheev, A. Y.; Vertogradov, L. S.; Yatsunenko, Y. A.] Joint Inst Nucl Res, Dubna, Russia. [Gavrilov, V.; Kiselevich, I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Boos, E. E.; Bunichev, V.; Dudko, L. V.; Karmanov, D.; Kuzmin, V. A.; Merkin, M.; Perfilov, M.] Moscow MV Lomonosov State Univ, Moscow, Russia. [Denisov, S. P.; Evdokimov, V. N.; Kozelov, A. V.; Lipaev, V. V.; Popov, A. V.; Prokopenko, N.; Razumov, I.; Shchukin, A. A.; Stoyanova, D. A.; Vasilyev, I. A.] Inst High Energy Phys, Protvino, Russia. [Alkhazov, G.; Lobodenko, A.; Neustroev, P.; Scheglov, Y.; Uvarov, L.; Uvarov, S.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Juste, A.] ICREA, Barcelona, Spain. [Juste, A.] IFAE, Barcelona, Spain. [Buszello, C. P.] Uppsala Univ, Uppsala, Sweden. [Bertram, I.; Borissov, G.; Burdin, S.; Fox, H.; Ratoff, P. N.; Ross, A.] Univ Lancaster, Lancaster LA1 4YB, England. [Beuselinck, R.; Davies, G.; Hays, J.; Jesik, R.; Jonsson, P.; Scanlon, T.] Univ London Imperial Coll Sci Technol & Med, London SW7 2AZ, England. [Agnew, J. P.; Ding, P. F.; Harder, K.; Head, T.; Hesketh, G.; McGivern, C. L.; Petridis, K.; Schwanenberger, C.; Soeldner-Rembold, S.; Suter, L.; Vesterinen, M.; Wyatt, T. R.; Zhao, T. G.] Univ Manchester, Manchester M13 9PL, Lancs, England. [Das, A.; Johns, K.; Lei, X.; Nayyar, R.; Varnes, E. W.] Univ Arizona, Tucson, AZ 85721 USA. [Ellison, J.; Heinson, A. P.; Joshi, J.; Li, L.] Univ Calif Riverside, Riverside, CA 92521 USA. [Adams, T.; Askew, A.; Bandurin, D. V.; Blessing, S.; Hoang, T.; Lee, W. M.; Wahl, H. D.] Florida State Univ, Tallahassee, FL 32306 USA. [Bagby, L.; Baldin, B.; Bartlett, J. F.; Bellantoni, L.; Bhat, P. C.; Boehnlein, A.; Bross, A.; Bu, X. B.; Buehler, M.; Casey, B. C. K.; Cihangir, S.; Cooke, M.; Cooper, W. E.; Denisov, D.; Desai, S.; Diehl, H. T.; Diesburg, M.; Elvira, V. D.; Fisk, H. E.; Fuess, S.; Ginther, G.; Greenlee, H.; Gruenendahl, S.; Gutierrez, G.; Herner, K.; Illingworth, R.; Ito, A. S.; Johnson, M.; Jonckheere, A.; Jung, A. W.; Khalatyan, N.; Li, Q. Z.; Lincoln, D.; Lipton, R.; Lyon, A. L.; Melnitchouk, A.; Penning, B.; Podstavkov, V. M.; Rominsky, M.; Rubinov, P.; Savage, G.; Verzocchi, M.; Wang, M. H. L. S.; Xie, Y.; Yamada, R.; Yasuda, T.; Ye, Z.; Yin, H.; Youn, S. W.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Adams, M.; Bazterra, V.; Gerber, C. E.; Varelas, N.] Univ Illinois, Chicago, IL 60607 USA. [Blazey, G.; Eads, M.; Feng, L.; Fortner, M.; Hedin, D.; Menezes, D.; Uzunyan, S.] No Illinois Univ, De Kalb, IL 60115 USA. [Schellman, H.; Welty-Rieger, L.] Northwestern Univ, Evanston, IL 60208 USA. [Evans, H.; Lammers, S.; Parua, N.; Price, D.; Van Kooten, R.; Williams, M. R. J.; Zieminska, D.] Indiana Univ, Bloomington, IN 47405 USA. [Parashar, N.] Purdue Univ Calumet, Hammond, IN 46323 USA. [Chan, K. M.; Hildreth, M. D.; Osta, J.; Ruchti, R.; Smirnov, D.; Warchol, J.; Wayne, M.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Hauptman, J. M.; Lee, S. W.] Iowa State Univ, Ames, IA 50011 USA. [Baringer, P.; Bean, A.; Chen, G.; Clutter, J.; Sekaric, J.; Wilson, G. W.] Univ Kansas, Lawrence, KS 66045 USA. [Atkins, S.; Sawyer, L.; Wobisch, M.] Louisiana Tech Univ, Ruston, LA 71272 USA. [Barberis, E.; Haley, J.; Wood, D. R.] Northeastern Univ, Boston, MA 02115 USA. [Alton, A.; Neal, H. A.; Qian, J.; Yu, J. M.; Zhou, B.; Zhu, J.] Univ Michigan, Ann Arbor, MI 48109 USA. [Brock, R.; Caughron, S.; Edmunds, D.; Fisher, W.; Geng, W.; Johnson, E.; Linnemann, J.; Schwienhorst, R.; Shaw, S.] Michigan State Univ, E Lansing, MI 48824 USA. [Bhatia, S.; Holzbauer, J. L.; Kraus, J.; Quinn, B.] Univ Mississippi, University, MS 38677 USA. [Bloom, K.; Claes, D.; DeVaughan, K.; Dominguez, A.; Katsanos, I.; Malik, S.; Snow, G. R.] Univ Nebraska, Lincoln, NE 68588 USA. [Gershtein, Y.] Rutgers State Univ, Piscataway, NJ 08855 USA. [Tully, C.] Princeton Univ, Princeton, NJ 08544 USA. [Iashvili, I.; Kharchilava, A.; Kumar, A.; Zennamo, J.] SUNY Buffalo, Buffalo, NY 14260 USA. [Demina, R.; Ferbel, T.; Garcia-Bellido, A.; Ginther, G.; Harel, A.; Petrillo, G.; Slattery, P.; Tsai, Y. -T.; Zielinski, M.] Univ Rochester, Rochester, NY 14627 USA. [Boline, D.; Chakrabarti, S.; Grannis, P. D.; Hobbs, J. D.; de Sa, R. Lopes; McCarthy, R.; Schamberger, R. D.; Tsybychev, D.; Ye, W.] SUNY Stony Brook, Stony Brook, NY 11794 USA. [Patwa, A.; Pleier, M. -A.; Snyder, S.; Yip, K.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Snow, J.] Langston Univ, Langston, OK 73050 USA. [Abbott, B.; Gutierrez, P.; Jayasinghe, A.; Severini, H.; Skubic, P.; Strauss, M.; Svoisky, P.] Univ Oklahoma, Norman, OK 73019 USA. [Hegab, H.; Khanov, A.; Rizatdinova, F.] Oklahoma State Univ, Stillwater, OK 74078 USA. [Cutts, D.; Heintz, U.; Jabeen, S.; Narain, M.; Parihar, V.; Partridge, R.] Brown Univ, Providence, RI 02912 USA. [Brandt, A.; Howley, I.; Pal, A.] Univ Texas Arlington, Arlington, TX 76019 USA. [Ilchenko, Y.; Kehoe, R.; Liu, H.] So Methodist Univ, Dallas, TX 75275 USA. [Chandra, A.; Corcoran, M.; Hogan, J.; Orduna, J.; Prewitt, M.] Rice Univ, Houston, TX 77005 USA. [Hirosky, R.; Li, H.; Mulhearn, M.; Nguyen, H. T.] Univ Virginia, Charlottesville, VA 22904 USA. [Watts, G.] Univ Washington, Seattle, WA 98195 USA. RP Abazov, VM (reprint author), Joint Inst Nucl Res, Dubna, Russia. RI Dudko, Lev/D-7127-2012; Sharyy, Viatcheslav/F-9057-2014; Lokajicek, Milos/G-7800-2014; Kupco, Alexander/G-9713-2014; Kozelov, Alexander/J-3812-2014; Lei, Xiaowen/O-4348-2014; Gutierrez, Phillip/C-1161-2011; Merkin, Mikhail/D-6809-2012; Li, Liang/O-1107-2015; Fisher, Wade/N-4491-2013; Santos, Angelo/K-5552-2012; Deliot, Frederic/F-3321-2014 OI Dudko, Lev/0000-0002-4462-3192; Sharyy, Viatcheslav/0000-0002-7161-2616; Lei, Xiaowen/0000-0002-2564-8351; Li, Liang/0000-0001-6411-6107; FU DOE; NSF (USA); CEA; CNRS/IN2P3 (France); MON; NRC KI; RFBR (Russia); CNPq; FAPERJ; FAPESP; FUNDUNESP (Brazil); DAE; DST (India); Colciencias (Colombia); CONACyT (Mexico); NRF (Korea); FOM (Netherlands); STFC; Royal Society (United Kingdom); MSMT; GACR (Czech Republic); BMBF; DFG (Germany); SFI (Ireland); Swedish Research Council (Sweden); CAS; CNSF (China) FX We thank the staffs at Fermilab and collaborating institutions, and we acknowledge support from the DOE and NSF (USA); CEA and CNRS/IN2P3 (France); MON, NRC KI, and RFBR (Russia); CNPq, FAPERJ, FAPESP, and FUNDUNESP (Brazil); DAE and DST (India); Colciencias (Colombia); CONACyT (Mexico); NRF (Korea); FOM (Netherlands); STFC and the Royal Society (United Kingdom); MSMT and GACR (Czech Republic); BMBF and DFG (Germany); SFI (Ireland); The Swedish Research Council (Sweden); and CAS and CNSF (China). NR 61 TC 8 Z9 8 U1 2 U2 21 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD OCT 21 PY 2013 VL 88 IS 7 AR 072008 DI 10.1103/PhysRevD.88.072008 PG 23 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 240OC UT WOS:000326105400001 ER PT J AU Kang, ZB Liu, XH Mantry, S Qiu, JW AF Kang, Zhong-Bo Liu, Xiaohui Mantry, Sonny Qiu, Jian-Wei TI Probing nuclear dynamics in jet production with a global event shape SO PHYSICAL REVIEW D LA English DT Article ID DEEP-INELASTIC SCATTERING; COLLINEAR EFFECTIVE THEORY; QUARK-GLUON PLASMA; COLOR GLASS CONDENSATE; RADIATIVE ENERGY-LOSS; TRANSVERSE-MOMENTUM; ROOT-S(NN)=2.76 TEV; PB COLLISIONS; QCD; HERA AB We study single jet production in electron-nucleus collisions e(-) + N-A -> J + X, using the 1-jettiness (tau(1)) global event shape. It inclusively quantifies the pattern of radiation in the final state, gives enhanced sensitivity to soft radiation at wide angles from the nuclear beam and final-state jet, and facilitates the resummation of large Sudakov logarithms associated with the veto on additional jets. Through their effect on the observed pattern of radiation, 1-jettiness can be a useful probe of nuclear parton distribution functions and power corrections from dynamical effects in the nuclear medium. This formalism allows for the standard jet shape analysis while simultaneously providing sensitivity to soft radiation at wide angles from the jet. We use a factorization framework for cross-sections differential in tau(1) and the transverse momentum (P-JT) and rapidity (y) of the jet, in the region tau(1) << P-JT. The restriction tau(1) << P-JT allows only soft radiation between the nuclear beam and jet directions, thereby acting as a veto on additional jets. This region is also insensitive to the details of the jet algorithm, allowing for better theoretical control over resummation, while providing enhanced sensitivity to nuclear medium effects. We give numerical results at leading twist, with resummation at the next-to-next-to-leading logarithmic level of accuracy, for a variety of nuclear targets. Such studies would be ideal for the electron-ion collider and the LHeC proposals for a future electron-ion collider, where a range of nuclear targets are planned. C1 [Kang, Zhong-Bo] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Liu, Xiaohui; Mantry, Sonny] Argonne Natl Lab, High Energy Div, Argonne, IL 60439 USA. [Liu, Xiaohui; Mantry, Sonny] Northwestern Univ, Dept Phys & Astron, Evanston, IL 60208 USA. [Qiu, Jian-Wei] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Qiu, Jian-Wei] SUNY Stony Brook, CN Yang Inst Theoret Phys, Stony Brook, NY 11794 USA. RP Kang, ZB (reprint author), Los Alamos Natl Lab, Div Theoret, POB 1663, Los Alamos, NM 87545 USA. RI Kang, Zhongbo/P-3645-2014; OI liu, xiaohui/0000-0002-7701-1205 FU U.S. Department of Energy [DE-AC02-05CH11231, DE-AC02-98CH10886, DE-AC02-06CH11357, DE-FG02-95ER40896, DE-FG02-08ER4153]; U.S. National Science Foundation [NSF-PHY-0705682] FX We thank Alberto Accardi and Frank Petriello for useful discussions and comments. This work was supported in part by the U.S. Department of Energy under Contracts No. DE-AC02-05CH11231 (Z.-B.K.), No. DE-AC02-98CH10886 (J.-W.Q.), No. DE-AC02-06CH11357 (X.L.) and Grants No. DE-FG02-95ER40896 (X.L.) and No. DE-FG02-08ER4153 (X.L.), and the U.S. National Science Foundation under Grant No. NSF-PHY-0705682 (S. M.). NR 84 TC 11 Z9 11 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD OCT 21 PY 2013 VL 88 IS 7 AR 074020 DI 10.1103/PhysRevD.88.074020 PG 29 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 240OC UT WOS:000326105400002 ER PT J AU Bergstrom, L Bringmann, T Cholis, I Hooper, D Weniger, C AF Bergstrom, Lars Bringmann, Torsten Cholis, Ilias Hooper, Dan Weniger, Christoph TI New Limits on Dark Matter Annihilation from Alpha Magnetic Spectrometer Cosmic Ray Positron Data SO PHYSICAL REVIEW LETTERS LA English DT Article ID SOLAR MODULATION; GALACTIC HALO; GAMMA-RAYS; PROPAGATION; CONSTRAINTS; PARTICLES; FRACTION; ELECTRONS; DENSITY; MODELS AB The Alpha Magnetic Spectrometer experiment onboard the International Space Station has recently provided cosmic ray electron and positron data with unprecedented precision in the range from 0.5 to 350 GeV. The observed rise in the positron fraction at energies above 10 GeV remains unexplained, with proposed solutions ranging from local pulsars to TeV-scale dark matter. Here, we make use of this high quality data to place stringent limits on dark matter with masses below similar to 300 GeV, annihilating or decaying to leptonic final states, essentially independent of the origin of this rise. We significantly improve on existing constraints, in some cases by up to 2 orders of magnitude. C1 [Bergstrom, Lars] Stockholm Univ, Oskar Klein Ctr Cosmoparticle Phys, Dept Phys, AlbaNova, SE-10691 Stockholm, Sweden. [Bringmann, Torsten] Univ Hamburg, Inst Theoret Phys 2, DE-22761 Hamburg, Germany. [Cholis, Ilias; Hooper, Dan] Fermilab Natl Accelerator Lab, Ctr Particle Astrophys, Batavia, IL 60510 USA. [Hooper, Dan] Univ Chicago, Dept Astron & Astrophys, Chicago, IL 60637 USA. [Weniger, Christoph] Univ Amsterdam, GRAPPA Inst, NL-1090 GL Amsterdam, Netherlands. RP Bergstrom, L (reprint author), Stockholm Univ, Oskar Klein Ctr Cosmoparticle Phys, Dept Phys, AlbaNova, SE-10691 Stockholm, Sweden. EM lbe@fysik.su.se; torsten.bringmann@desy.de; cholis@fnal.gov; dhooper@fnal.gov; c.weniger@uva.nl OI Bringmann, Torsten/0000-0002-0339-8144 FU Swedish Research Council [621-2009-3915]; German Research Foundation (DFG) [BR 3954/1-1]; U.S. Department of Energy FX This work makes use of SCIPY [78], MINUIT [79], and MATPLOTLIB [80]. The research of L. B. was carried out under Swedish Research Council (VR) Contract No. 621-2009-3915. T. B. acknowledges support from the German Research Foundation (DFG) through the Emmy Noether Grant No. BR 3954/1-1. I. C., C. W., and D. H. thank the Kavli Institute for Theoretical Physics in Santa Barbara, California, for their kind hospitality. This work has been supported by the U.S. Department of Energy. NR 86 TC 105 Z9 105 U1 0 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 21 PY 2013 VL 111 IS 17 AR 171101 DI 10.1103/PhysRevLett.111.171101 PG 6 WC Physics, Multidisciplinary SC Physics GA 241EB UT WOS:000326148100002 PM 24206472 ER PT J AU Qu, DX Roberts, SK Chapline, GF AF Qu, Dong-Xia Roberts, Sarah K. Chapline, George F. TI Observation of Huge Surface Hole Mobility in the Topological Insulator Bi0.91Sb0:09 (111) SO PHYSICAL REVIEW LETTERS LA English DT Article ID SINGLE DIRAC CONE; STATES; BI2SE3; BI2TE3 AB We report the first direct measurement of transport properties of surface states in the topological insulator Bi0.91Sb0.09 (111) from the weak-field Hall effect and Shubnikov-de Haas oscillations. We find that the holelike surface band displays an unexpectedly high mobility 23 000-85 000 cm(2)/Vs, which is the highest mobility so far reported in bismuth-based topological insulators. This result provides the first quantitative assessment of the effect of alloy disorder on the mobility of surface states in topological insulators. We show that the 9% alloy disorder decreases the mobility of surface states by a factor of less than 2.3. C1 [Qu, Dong-Xia; Roberts, Sarah K.; Chapline, George F.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Qu, DX (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM dxqu@lbl.gov FU LDRD from Lawrence Livermore National Laboratory [12-ERD-027] FX We would like to thank H.-J. Zhang and S.-C. Zhang for helpful discussions. The high magnetic field measurements were performed at the National High Magnetic Field Laboratory, Tallahassee, Florida. We would like to thank D. Graf, A. Suslov, and G. S. Boebinger for assistance with the experimental measurements. This work was supported by LDRD (12-ERD-027) from Lawrence Livermore National Laboratory. NR 28 TC 5 Z9 5 U1 3 U2 31 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 21 PY 2013 VL 111 IS 17 AR 176801 DI 10.1103/PhysRevLett.111.176801 PG 5 WC Physics, Multidisciplinary SC Physics GA 241EB UT WOS:000326148100005 PM 24206511 ER PT J AU Linville, JL Rodriguez, M Land, M Syed, MH Engle, NL Tschaplinski, TJ Mielenz, JR Cox, CD AF Linville, Jessica L. Rodriguez, Miguel, Jr. Land, Miriam Syed, Mustafa H. Engle, Nancy L. Tschaplinski, Timothy J. Mielenz, Jonathan R. Cox, Chris D. TI Industrial Robustness: Understanding the Mechanism of Tolerance for the Populus Hydrolysate-Tolerant Mutant Strain of Clostridium thermocellum SO PLOS ONE LA English DT Article ID ETHANOLOGENIC ESCHERICHIA-COLI; DEGRADATION-PRODUCTS; BACILLUS-SUBTILIS; SACCHAROMYCES-CEREVISIAE; TRANSCRIPTIONAL ANALYSIS; SIGMA FACTORS; CORN STOVER; FERMENTATION; BIOMASS; PRETREATMENT AB Background: An industrially robust microorganism that can efficiently degrade and convert lignocellulosic biomass into ethanol and next-generation fuels is required to economically produce future sustainable liquid transportation fuels. The anaerobic, thermophilic, cellulolytic bacterium Clostridium thermocellum is a candidate microorganism for such conversions but it, like many bacteria, is sensitive to potential toxic inhibitors developed in the liquid hydrolysate produced during biomass processing. Microbial processes leading to tolerance of these inhibitory compounds found in the pretreated biomass hydrolysate are likely complex and involve multiple genes. Methodology/Principal Findings: In this study, we developed a 17.5% v/v Populus hydrolysate tolerant mutant strain of C. thermocellum by directed evolution. The genome of the wild type strain, six intermediate population samples and seven single colony isolates were sequenced to elucidate the mechanism of tolerance. Analysis of the 224 putative mutations revealed 73 high confidence mutations. A longitudinal analysis of the intermediate population samples, a pan-genomic analysis of the isolates, and a hotspot analysis revealed 24 core genes common to all seven isolates and 8 hotspots. Genetic mutations were matched with the observed phenotype through comparison of RNA expression levels during fermentation by the wild type strain and mutant isolate 6 in various concentrations of Populus hydrolysate (0%, 10%, and 17.5% v/v). Conclusion/Significance: The findings suggest that there are multiple mutations responsible for the Populus hydrolysate tolerant phenotype resulting in several simultaneous mechanisms of action, including increases in cellular repair, and altered energy metabolism. To date, this study provides the most comprehensive elucidation of the mechanism of tolerance to a pretreated biomass hydrolysate by C. thermocellum. These findings make important contributions to the development of industrially robust strains of consolidated bioprocessing microorganisms. C1 [Linville, Jessica L.; Cox, Chris D.] Univ Tennessee, Dept Civil & Environm Engn, Knoxville, TN 37996 USA. [Linville, Jessica L.; Rodriguez, Miguel, Jr.; Land, Miriam; Syed, Mustafa H.; Engle, Nancy L.; Tschaplinski, Timothy J.; Mielenz, Jonathan R.; Cox, Chris D.] Oak Ridge Natl Lab, Bioenergy Sci Ctr, Oak Ridge, TN USA. [Rodriguez, Miguel, Jr.; Syed, Mustafa H.; Engle, Nancy L.; Tschaplinski, Timothy J.; Mielenz, Jonathan R.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN USA. [Cox, Chris D.] Univ Tennessee, Inst Secure & Sustainable Environm, Knoxville, TN USA. RP Cox, CD (reprint author), Univ Tennessee, Dept Civil & Environm Engn, Knoxville, TN 37996 USA. EM ccox9@utk.edu RI Land, Miriam/A-6200-2011; OI Land, Miriam/0000-0001-7102-0031; Tschaplinski, Timothy/0000-0002-9540-6622; Engle, Nancy/0000-0003-0290-7987 FU BioEnergy Science Center, a Department of Energy Bioenergy Research Center; Office of Biological and Environmental Research in the Department of Energy Office of Science; Institute for a Secure and Sustainable Environment at the University of Tennessee; DOE [DE-AC05-00OR22725] FX This research was supported by the BioEnergy Science Center, a Department of Energy Bioenergy Research Center supported by the Office of Biological and Environmental Research in the Department of Energy Office of Science. Additional support was provided by the Institute for a Secure and Sustainable Environment at the University of Tennessee. Oak Ridge National Laboratory is managed by UT-Battelle, LLC, for the DOE under Contract DE-AC05-00OR22725. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 65 TC 8 Z9 8 U1 1 U2 20 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD OCT 21 PY 2013 VL 8 IS 10 AR UNSP e78829 DI 10.1371/journal.pone.0078829 PG 16 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 239NN UT WOS:000326032600112 PM 24205326 ER PT J AU Neupane, M Basak, S Alidoust, N Xu, SY Liu, C Belopolski, I Bian, G Xiong, J Ji, H Jia, S Mo, SK Bissen, M Severson, M Lin, H Ong, NP Durakiewicz, T Cava, RJ Bansil, A Hasan, MZ AF Neupane, M. Basak, S. Alidoust, N. Xu, S. -Y. Liu, Chang Belopolski, I. Bian, G. Xiong, J. Ji, H. Jia, S. Mo, S. -K. Bissen, M. Severson, M. Lin, H. Ong, N. P. Durakiewicz, T. Cava, R. J. Bansil, A. Hasan, M. Z. TI Oscillatory surface dichroism of the insulating topological insulator Bi2Te2Se SO PHYSICAL REVIEW B LA English DT Article ID ANGLE-RESOLVED PHOTOEMISSION; CIRCULAR-DICHROISM; PHASE AB Using circular dichroism-angle resolved photoemission spectroscopy, we report a study of the effect of angular momentum transfer between polarized photons and topological surface states on the surface of the insulating topological insulator Bi2Te2Se. The photoelectron dichroism is found to be strongly modulated by the frequency of the helical photons including a dramatic sign flip. Our results suggest that the observed dichroism and its sign flip are consequences of strong coupling between the photon field and the spin-orbit nature of the Dirac modes on the surface. Our studies reveal the intrinsic dichroic behavior of topological surface states and point toward the potential utility of bulk insulating topological insulators in opto-spintronics device applications. C1 [Neupane, M.; Alidoust, N.; Xu, S. -Y.; Liu, Chang; Belopolski, I.; Bian, G.; Xiong, J.; Ong, N. P.; Hasan, M. Z.] Princeton Univ, Joseph Henry Labs, Princeton, NJ 08544 USA. [Neupane, M.; Alidoust, N.; Xu, S. -Y.; Liu, Chang; Belopolski, I.; Bian, G.; Xiong, J.; Ong, N. P.; Hasan, M. Z.] Princeton Univ, Dept Phys, Princeton, NJ 08544 USA. [Basak, S.; Lin, H.; Bansil, A.] Northeastern Univ, Dept Phys, Boston, MA 02115 USA. [Ji, H.; Jia, S.; Cava, R. J.] Princeton Univ, Dept Chem, Princeton, NJ 08544 USA. [Mo, S. -K.] Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94305 USA. [Bissen, M.; Severson, M.] Univ Wisconsin, Ctr Synchrotron Radiat, Stoughton, WI 53589 USA. [Durakiewicz, T.] Los Alamos Natl Lab, Condensed Matter & Magnet Sci Grp, Los Alamos, NM 87545 USA. [Hasan, M. Z.] Princeton Univ, Princeton Ctr Complex Mat, Princeton, NJ 08544 USA. RP Hasan, MZ (reprint author), Princeton Univ, Joseph Henry Labs, Princeton, NJ 08544 USA. EM mzhasan@princeton.edu RI HASAN, M. Zahid/D-8237-2012; Ji, Huiwen/O-5145-2014; Mo, Sung-Kwan/F-3489-2013; Bian, Guang/C-5182-2016; Lin, Hsin/F-9568-2012 OI Mo, Sung-Kwan/0000-0003-0711-8514; Bian, Guang/0000-0001-7055-2319; Lin, Hsin/0000-0002-4688-2315 FU DARPA Meso Grant [N66001-11-1-4110]; Department of Energy, Office of Basic Energy Sciences, Division of Material Sciences; A.P. Sloan Foundation; [NSF/DMR-1006492] FX This work was primarily supported by DARPA Meso Grant No. N66001-11-1-4110. The use of Synchrotron Radiation Center (SRC) was supported by NSF DMR-0537588 under the external user agreement. We acknowledge Peter Rise-borough and Luca Perfetti for discussions. T. D. at LANL acknowledges support from Department of Energy, Office of Basic Energy Sciences, Division of Material Sciences. M.Z.H. acknowledges Visiting Scientist support from LBNL and partial support from NSF/DMR-1006492 and A.P. Sloan Foundation. NR 35 TC 15 Z9 15 U1 2 U2 57 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 21 PY 2013 VL 88 IS 16 AR 165129 DI 10.1103/PhysRevB.88.165129 PG 8 WC Physics, Condensed Matter SC Physics GA 240IC UT WOS:000326087800005 ER PT J AU Scheinker, A Pang, XY Rybarcyk, L AF Scheinker, Alexander Pang, Xiaoying Rybarcyk, Larry TI Model-independent particle accelerator tuning SO PHYSICAL REVIEW SPECIAL TOPICS-ACCELERATORS AND BEAMS LA English DT Article AB We present a new model-independent dynamic feedback technique, rotation rate tuning, for automatically and simultaneously tuning coupled components of uncertain, complex systems. The main advantages of the method are: (1) it has the ability to handle unknown, time-varying systems, (2) it gives known bounds on parameter update rates, (3) we give an analytic proof of its convergence and its stability, and (4) it has a simple digital implementation through a control system such as the experimental physics and industrial control system (EPICS). Because this technique is model independent it may be useful as a realtime, in-hardware, feedback-based optimization scheme for uncertain and time-varying systems. In particular, it is robust enough to handle uncertainty due to coupling, thermal cycling, misalignments, and manufacturing imperfections. As a result, it may be used as a fine-tuning supplement for existing accelerator tuning/control schemes. We present multiparticle simulation results demonstrating the scheme's ability to simultaneously adaptively adjust the set points of 22 quadrupole magnets and two rf buncher cavities in the Los Alamos Neutron Science Center (LANSCE) Linear Accelerator's transport region, while the beam properties and rf phase shift are continuously varying. The tuning is based only on beam current readings, without knowledge of particle dynamics. We also present an outline of how to implement this general scheme in software for optimization, and in hardware for feedback-based control/tuning, for a wide range of systems. C1 [Scheinker, Alexander; Pang, Xiaoying; Rybarcyk, Larry] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Scheinker, A (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM ascheink@lanl.gov; xpang@lanl.gov; lrybarcyk@lanl.gov FU Los Alamos National Laboratory FX This research was supported by Los Alamos National Laboratory. NR 18 TC 5 Z9 5 U1 0 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-4402 J9 PHYS REV SPEC TOP-AC JI Phys. Rev. Spec. Top.-Accel. Beams PD OCT 21 PY 2013 VL 16 IS 10 AR 102803 DI 10.1103/PhysRevSTAB.16.102803 PG 10 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA 241EO UT WOS:000326149400001 ER PT J AU Xu, P Kang, LL Mack, NH Schanze, KS Han, XJ Wang, HL AF Xu, Ping Kang, Leilei Mack, Nathan H. Schanze, Kirk S. Han, Xijiang Wang, Hsing-Lin TI Mechanistic understanding of surface plasmon assisted catalysis on a single particle: cyclic redox of 4-aminothiophenol SO SCIENTIFIC REPORTS LA English DT Article ID ENHANCED RAMAN-SPECTROSCOPY; SCATTERING SPECTROSCOPY; P-AMINOTHIOPHENOL; AG; AU; P,P'-DIMERCAPTOAZOBENZENE; NANOPARTICLES; 4,4'-DIMERCAPTOAZOBENZENE; 4-NITROBENZENETHIOL; PHOTOREDUCTION AB Surface plasmon assisted catalysis (SPAC) reactions of 4-aminothiophenol (4ATP) to and back from 4,4'-dimercaptoazobenzene (DMAB) have been investigated by single particle surface enhanced Raman spectroscopy, using a self-designed gas flow cell to control the reductive/oxidative environment over the reactions. Conversion of 4ATP into DMAB is induced by energy transfer (plasmonic heating) from surface plasmon resonance to 4ATP, where O-2 (as an electron acceptor) is essential and H2O (as a base) can accelerate the reaction. In contrast, hot electron (from surface plasmon decay) induction drives the reverse reaction of DMAB to 4ATP, where H2O (or H-2) acts as the hydrogen source. More interestingly, the cyclic redox between 4ATP and DMAB by SPAC approach has been demonstrated. This SPAC methodology presents a unique platform for studying chemical reactions that are not possible under standard synthetic conditions. C1 [Xu, Ping; Kang, Leilei; Han, Xijiang] Harbin Inst Technol, Dept Chem, Harbin 150001, Peoples R China. [Xu, Ping; Mack, Nathan H.; Wang, Hsing-Lin] Los Alamos Natl Lab, Div Chem, Los Alamos, NM 87545 USA. [Schanze, Kirk S.] Univ Florida, Dept Chem, Gainesville, FL 32611 USA. RP Xu, P (reprint author), Harbin Inst Technol, Dept Chem, Harbin 150001, Peoples R China. EM pxu@hit.edu.cn; hanxijiang@hit.edu.cn; hwang@lanl.gov RI Xu, Ping/I-1910-2013; Schanze, Kirk/A-7200-2009 OI Xu, Ping/0000-0002-1516-4986; Schanze, Kirk/0000-0003-3342-4080 FU NSFC [21203045, 21101041, 21003029, 21071037, 91122002]; Fundamental Research Funds for the Central Universities [HIT.NSRIF. 2010065, 2011017, HIT.BRETIII. 201223]; 9th Thousand Foreign Experts Program; Laboratory Directed Research and Development (LDRD) fund under the DOE FX This work was supported by NSFC (No. 21203045, 21101041, 21003029, 21071037, 91122002), Fundamental Research Funds for the Central Universities (No. HIT.NSRIF. 2010065 and 2011017, and HIT.BRETIII. 201223), the 9th Thousand Foreign Experts Program, and Director's Postdoctoral Fellow from LANL. HLW acknowledges the financial support from the Laboratory Directed Research and Development (LDRD) fund under the auspices of DOE. Synthesis and characterization of nanostructured metals is supported by Basic Energy Science (BES), Biomolecular Materials Program, Materials Sciences and Engineering Division. PX would like to thank Prof. Mengtao Sun and Dr. Cunku Dong for the DFT calculations. NR 25 TC 76 Z9 76 U1 9 U2 152 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD OCT 21 PY 2013 VL 3 AR 2997 DI 10.1038/srep02997 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 237JQ UT WOS:000325866100009 PM 24141289 ER PT J AU Maxson, JM Bazarov, IV Wan, W Padmore, HA Coleman-Smith, CE AF Maxson, J. M. Bazarov, I. V. Wan, W. Padmore, H. A. Coleman-Smith, C. E. TI Fundamental photoemission brightness limit from disorder induced heating SO NEW JOURNAL OF PHYSICS LA English DT Article ID NEGATIVE ELECTRON-AFFINITY; PHOTOCATHODES; PLASMA AB We determine the limit of the lowest achievable photoemitted electron temperature, and therefore the maximum achievable electron brightness, from unstructured photoemitting materials producing dense relativistic or nonrelativistic photoelectron beams. The limit is given by electron heating that occurs just after emission into vacuum, and is due to poorly screened Coulomb interactions equivalent to disorder induced heating seen in ultracold neutral plasmas. We first show that traditional analytic methods of Coulomb collisions fail for the calculation of this strongly coupled heating. Instead, we employ an N-body tree algorithm to compute the universal scaling of the disorder induced heating in fully contained bunches, and show it to agree well with a simple model utilizing the tabulated correlated energy of one component plasmas. We also present simulations for beams undergoing Coulomb explosion at the photoemitter, and demonstrate that both the temperature growth and subsequent cooling must be characterized by correlated effects, as well as correlation-frozen dynamics. In either case, the induced temperature is found to be of several meV for typical photoinjector beam densities, a significant fraction of the intrinsic beam temperature of the coldest semiconductor photocathodes. Thus, we expect disorder induced heating to become a major limiting factor in the next generation of photoemission sources delivering dense bunches and employing ultra-cold photoemitters. C1 [Maxson, J. M.; Bazarov, I. V.] Cornell Univ, Cornell Lab Accelerator Based Sci & Educ, Ithaca, NY 14853 USA. [Wan, W.; Padmore, H. A.] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Coleman-Smith, C. E.] Duke Univ, Dept Phys, Durham, NC 27708 USA. RP Maxson, JM (reprint author), Cornell Univ, Cornell Lab Accelerator Based Sci & Educ, Ithaca, NY 14853 USA. EM jmm586@cornell.edu FU National Science Foundation [DGE-0707428]; Department of Energy [DE-SC0003965]; Director, Office of Science, Office of Basic Energy Sciences of the US Department of Energy; [DE-AC02-05CH11231]; [KC0407-LSJNT-I0013]; [DE-SC0005713] FX The authors thank two anonymous reviewers for helpful suggestions that clarified the presentation of the work. The authors also thank Joshua Barnes, the original author of the treecode package modified for use in this work. This work was supported by the National Science Foundation grant no. DGE-0707428, and by the Department of Energy grant no. DE-SC0003965. This work was also supported by the Director, Office of Science, Office of Basic Energy Sciences of the US Department of Energy, under contract numbers DE-AC02-05CH11231, KC0407-LSJNT-I0013 and DE-SC0005713. NR 23 TC 11 Z9 11 U1 1 U2 11 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1367-2630 J9 NEW J PHYS JI New J. Phys. PD OCT 21 PY 2013 VL 15 AR 103024 DI 10.1088/1367-2630/15/10/103024 PG 13 WC Physics, Multidisciplinary SC Physics GA 237CX UT WOS:000325846900001 ER PT J AU Ryan, SD Sokolov, A Berlyand, L Aranson, IS AF Ryan, Shawn D. Sokolov, Andrey Berlyand, Leonid Aranson, Igor S. TI Correlation properties of collective motion in bacterial suspensions SO NEW JOURNAL OF PHYSICS LA English DT Article ID DIFFUSION AB The study of collective motion in bacterial suspensions has been of significant recent interest. To better understand the non-trivial spatio-temporal correlations emerging in the course of collective swimming in suspensions of motile bacteria, a simple model is employed: a bacterium is represented as a force dipole with size, through the use of a short-range repelling potential, and shape. The model emphasizes two fundamental mechanisms: dipolar hydrodynamic interactions and short-range bacterial collisions. Using direct particle simulations validated by a dedicated experiment, we show that changing the swimming speed or concentration alters the time scale of sustained collective motion, consistent with experiment. Also, the correlation length in the collective state is almost constant as concentration and swimming speed change even though increasing each greatly increases the input of energy to the system. We demonstrate that the particle shape is critical for the onset of collective effects. In addition, new experimental results are presented illustrating the onset of collective motion with an ultrasound technique. This work exemplifies the delicate balance between various physical mechanisms governing collective motion in bacterial suspensions and provides important insights into its mesoscopic nature. C1 [Ryan, Shawn D.; Berlyand, Leonid] Penn State Univ, Dept Math, University Pk, PA 16802 USA. [Ryan, Shawn D.; Sokolov, Andrey; Aranson, Igor S.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Aranson, Igor S.] Northwestern Univ, Evanston, IL 60202 USA. RP Ryan, SD (reprint author), Penn State Univ, Dept Math, University Pk, PA 16802 USA. EM ryan@math.psu.edu OI Ryan, Shawn/0000-0003-2468-1827 FU US DOE BES, Division of Materials Science and Engineering [DE AC02-06CH11357]; NIH [1R01GM104978-01]; DOE grant [DE-FG02-08ER25862] FX AS and ISA were supported by the US DOE BES, Division of Materials Science and Engineering, under contract no. DE AC02-06CH11357 (simulations), and ISA was supported by the NIH grant 1R01GM104978-01 (modeling/experiment). The work of LB was supported by the NIH grant 1R01GM104978-01. The work of SDR was supported by the DOE grant DE-FG02-08ER25862. NR 28 TC 10 Z9 10 U1 1 U2 22 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1367-2630 J9 NEW J PHYS JI New J. Phys. PD OCT 21 PY 2013 VL 15 AR 105021 DI 10.1088/1367-2630/15/10/105021 PG 18 WC Physics, Multidisciplinary SC Physics GA 237CV UT WOS:000325846700004 ER PT J AU Bowen, JD Huang, Q Ellin, JR Lee, TC Shrestha, U Gullberg, GT Seo, Y AF Bowen, Jason D. Huang, Qiu Ellin, Justin R. Lee, Tzu-Cheng Shrestha, Uttam Gullberg, Grant T. Seo, Youngho TI Design and performance evaluation of a 20-aperture multipinhole collimator for myocardial perfusion imaging applications SO PHYSICS IN MEDICINE AND BIOLOGY LA English DT Article ID ULTRA-HIGH-RESOLUTION; MULTI-PINHOLE SPECT; CORONARY-ARTERY-DISEASE; SMALL ANIMAL SPECT; RECONSTRUCTION ALGORITHMS; SYNTHETIC COLLIMATION; EMISSION TOMOGRAPHY; SPATIAL-RESOLUTION; COST-EFFECTIVENESS; SYSTEM AB Single photon emission computed tomography (SPECT) myocardial perfusion imaging remains a critical tool in the diagnosis of coronary artery disease. However, after more than three decades of use, photon detection efficiency remains poor and unchanged. This is due to the continued reliance on parallel-hole collimators first introduced in 1964. These collimators possess poor geometric efficiency. Here we present the performance evaluation results of a newly designed multipinhole collimator with 20 pinhole apertures (PH20) for commercial SPECT systems. Computer simulations and numerical observer studies were used to assess the noise, bias and diagnostic imaging performance of a PH20 collimator in comparison with those of a low energy high resolution (LEHR) parallel-hole collimator. Ray-driven projector/backprojector pairs were used to model SPECT imaging acquisitions, including simulation of noiseless projection data and performing MLEM/OSEM image reconstructions. Poisson noise was added to noiseless projections for realistic projection data. Noise and bias performance were investigated for five mathematical cardiac and torso (MCAT) phantom anatomies imaged at two gantry orbit positions (19.5 and 25.0 cm). PH20 and LEHR images were reconstructed with 300 MLEM iterations and 30 OSEM iterations (ten subsets), respectively. Diagnostic imaging performance was assessed by a receiver operating characteristic (ROC) analysis performed on a single MCAT phantom; however, in this case PH20 images were reconstructed with 75 pixel-based OSEM iterations (four subsets). Four PH20 projection views from two positions of a dual-head camera acquisition and 60 LEHR projections were simulated for all studies. At uniformly-imposed resolution of 12.5 mm, significant improvements in SNR and diagnostic sensitivity (represented by the area under the ROC curve, or AUC) were realized when PH20 collimators are substituted for LEHR parallel-hole collimators. SNR improves by factors of 1.94-2.34 for the five patient anatomies and two orbital positions studied. For the ROC analysis the PH20 AUC is larger than the LEHR AUC with a p-value of 0.0067. Bias performance, however, decreases with the use of PH20 collimators. Systematic analyses showed PH20 collimators present improved diagnostic imaging performance over LEHR collimators, requiring only collimator exchange on existing SPECT cameras for their use. C1 [Bowen, Jason D.; Ellin, Justin R.; Lee, Tzu-Cheng; Shrestha, Uttam; Gullberg, Grant T.; Seo, Youngho] Univ Calif San Francisco, Dept Radiol & Biomed Imaging, Phys Res Lab, San Francisco, CA 94143 USA. [Huang, Qiu] Shanghai Jiao Tong Univ, Shanghai 200030, Peoples R China. [Gullberg, Grant T.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Radiotracer Dev & Imaging Technol, Berkeley, CA 94720 USA. [Seo, Youngho] Univ Calif San Francisco, Dept Radiat Oncol, San Francisco, CA USA. RP Bowen, JD (reprint author), Univ Calif San Francisco, Dept Radiol & Biomed Imaging, Phys Res Lab, San Francisco, CA 94143 USA. EM youngho.seo@ucsf.edu FU National Heart, Lung and Blood Institute [R21 HL083073, R01 HL050663]; National Institute of Biomedical Imaging and Bioengineering [R01 EB012965] FX We thank Dr George Sayre for helpful discussions. This work was supported in part by National Heart, Lung and Blood Institute under grant #R21 HL083073 (JDB and YS) and grant #R01 HL050663 (JE, US, GTG, and YS), and National Institute of Biomedical Imaging and Bioengineering under grant R01 EB012965 (T-CL and YS). NR 49 TC 8 Z9 9 U1 1 U2 6 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0031-9155 J9 PHYS MED BIOL JI Phys. Med. Biol. PD OCT 21 PY 2013 VL 58 IS 20 BP 7209 EP 7226 DI 10.1088/0031-9155/58/20/7209 PG 18 WC Engineering, Biomedical; Radiology, Nuclear Medicine & Medical Imaging SC Engineering; Radiology, Nuclear Medicine & Medical Imaging GA 228FY UT WOS:000325172500012 PM 24061162 ER PT J AU Aad, G Abajyan, T Abbott, B Abdallah, J Khalek, SA Abdelalim, AA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Addy, TN Adelman, J Adomeit, S Adye, T Aefsky, S Agatonovic-Jovin, T Aguilar-Saavedra, JA Agustoni, M Ahlen, SP Ahles, F Ahmad, A Ahsan, M Aielli, G Akesson, TPA Akimoto, G Akimov, AV Alam, MA Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alessandria, F Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Aliev, M Alimonti, G Alison, J Allbrooke, BMM Allison, LJ Allport, PP Allwood-Spiers, SE Almond, J Aloisio, A Alon, R Alonso, A Alonso, F Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Coutinho, YA Amelung, C Ammosov, VV Dos Santos, SPA Amorim, A Amoroso, S Amram, N Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Anduaga, XS Angelidakis, S Anger, P Angerami, A Anghinolfi, E Anisenkov, AV Anjos, N Annovi, A Antonaki, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Apolle, R Arabidze, G Aracena, I Arai, Y Arce, ATH Arfaoui, S Arguin, JF Argyropoulos, S Arik, E Arik, M Armbruster, AJ Arnaez, O Arnal, V Artamonov, A Artoni, G Arutinov, D Asai, S Asbah, N Ask, S Asman, B Asquith, L Assamagan, K Astalos, R Astbury, A Atkinson, M Auerbach, B Auge, E Augsten, K Aurousseau, M Avolio, G Axen, D Azuelos, G Azuma, Y Baak, MA Bacci, C Bach, AM Bachacou, H Bachas, K Backes, M Backhaus, M Mayes, JB Badescu, E Bagiacchi, P Bagnaia, P Bai, Y Bailey, DC Bain, T Baines, JT Baker, OK Baker, S Balek, P Balli, F Banas, E Banerjee, P Banerjee, S Banfi, D Bangert, A Bansal, V Bansil, HS Barak, L Baranov, SP Barber, T Barberio, EL Barberis, D 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O Bieniek, SP Bierwagen, K Biesiada, J Biglietti, M Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Bittner, B Black, CW Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blazek, T Bloch, I Blocker, C Blocki, J Blum, W Blumenschein, U Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Boddy, CR Boehler, M Boek, J Boek, TT Boelaert, N Bogaerts, JA Bogdanchikov, AG Bogouch, A Bohm, C Bohm, J Boisvert, V Bold, T Boldea, V Bolnet, NM Bomben, M Bona, M Boonekamp, M Bordoni, S Borer, C Borisov, A Borissov, G Born, M Borroni, S Bortfeldt, J Bortolotto, V Bos, K Boscherini, D Bosman, M Boterenbrood, H Bouchami, J Boudreau, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boutouil, S Boveia, A Boyd, J Boyko, IR Bozovic-Jelisavcic, I Bracinik, J Branchini, P Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Brazzale, SF Brelier, B Bremer, J Brendlinger, K Brenner, R Bressler, S Bristow, TM Britton, D Brochu, FM Brock, I Brock, R Broggi, F Bromberg, C Bronner, 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Zaidan, R. Zaitsev, A. M. Zambito, S. Zanello, L. Zanzi, D. Zaytsev, A. Zeitnitz, C. Zeman, M. Zemla, A. Zenin, . Zenis, T. Zerwas, D. della Porta, G. Zevi Zhang, D. Zhang, H. Zhang, J. Zhang, L. Zhang, X. Zhang, Z. Zhao, Z. Zhemchugov, A. Zhong, J. Zhou, B. Zhou, N. Zhou, Y. Zhu, C. G. Zhu, H. Zhu, J. Zhu, Y. Zhuang, X. Zibell, A. Zieminska, D. Zimin, N. I. Zimmermann, C. Zimmermann, R. Zimmermann, S. Zimmermann, S. Zinonos, Z. Ziolkowski, M. Zitoun, R. Zivkovic, L. Zmouchko, V. V. Zobernig, G. Zoccoli, A. zur Nedden, M. Zutshi, V. Zwalinski, L. CA ATLAS Collaboration TI Dynamics of isolated-photon plus jet production in pp collisions at root s=7 TeV with the ATLAS detector SO NUCLEAR PHYSICS B LA English DT Article DE QCD; Photon; Jet ID FRAGMENTATION; LHC; PROTON; BOSON; MODEL AB The dynamics of isolated-photon plus jet production in pp collisions at a centre-of-mass energy of 7 TeV has been studied with the ATLAS detector at the LHC using an integrated luminosity of 37 pb(-1). Measurements of isolated-photon plus jet bin-averaged cross sections are presented as functions of photon transverse energy, jet transverse momentum and jet rapidity. In addition, the bin-averaged cross sections as functions of the difference between the azimuthal angles of the photon and the jet, the photon jet invariant mass and the scattering angle in the photon jet centre-of-mass frame have been measured. Next-to-leading-order QCD calculations are compared to the measurements and provide a good description of the data, except for the case of the azimuthal opening angle. (C) 2013 CERN. Published by Elsevier B.V. All rights reserved. C1 [Jackson, P.; Soni, N.] Univ Adelaide, Sch Chem & Phys, Adelaide, SA, Australia. [Edson, W.; Ernst, J.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Chan, K.; Gingrich, D. M.; Moore, R. W.; Pinfold, J. L.; Saddique, A.; Sbrizzi, A.; Subramania, Hs.; Vague, F. Vives] Univ Alberta, Dept Phys, Edmonton, AB, Canada. 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[Beddall, A. J.; Beddall, A.; Bingul, A.] Gaziantep Univ, Dept Engn Phys, Gaziantep, Turkey. [Bellagamba, L.; Bindi, M.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; Corradi, M.; De Castro, S.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Giacobbe, B.; Grafstroem, P.; Jha, M. K.; Massa, I.; Mengarelli, A.; Monzani, S.; Negrini, M.; Piccinini, M.; Polini, A.; Rinaldi, L.; Romano, M.; Sbarra, C.; Semprini-Cesari, N.; Spighi, R.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, INFN Sez Bologna, Bologna, Italy. [Bindi, M.; Caforio, D.; De Castro, S.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Grafstroem, P.; Massa, I.; Mengarelli, A.; Monzani, S.; Piccinini, M.; Romano, M.; Semprini-Cesari, N.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, Dipartimento Fis & Astron, Bologna, Italy. [Abajyan, T.; Arutinov, D.; Backhaus, M.; Bechtle, P.; Brock, I.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Ehrenfeld, W.; Gaycken, G.; Geich-Gimbel, Ch.; Glatzer, J.; Gonella, L.; Haefner, P.; Havranek, M.; Hellmich, D.; Hillert, S.; Huegging, F.; Janssen, J.; Khoriauli, G.; Koevesarki, P.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lapoire, C.; Lehmacher, M.; Leyko, A. M.; Liebal, J.; Limbach, C.; Loddenkoetter, T.; Mazur, M.; Moeser, N.; Mueller, K.; Nanava, G.; Nattermann, T.; Nuncio-Quiroz, A. -E.; Pohl, D.; Psoroulas, S.; Sarrazin, B.; Schaepe, S.; Schultens, M. J.; Schwindt, T.; Scutti, F.; Stillings, J. A.; Therhaag, J.; Tsung, J. -W.; Uchida, K.; Uhlenbrock, M.; Urquijo, P.; Vogel, A.; von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, R.; Wiik-Fuchs, L. A. M.; Wong, K. H. Yau; Zimmermann, R.; Zimmermann, S.] Univ Bonn, Inst Phys, Bonn, Germany. [Ahlen, S. P.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, Boston, MA 02215 USA. [Aefsky, S.; Amelung, C.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Daya-Ishmukhametova, R. K.; Fitzgerald, E. A.; Gozpinar, S.; Pomeroy, D.; Sciolla, G.; Zambito, S.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Amaral Coutinho, Y.; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio De Janeiro COPPE EE IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; Manhaes de Andrade Filho, L.] Fed Univ Juiz de Fora UFJF, Juiz De Fora, Brazil. [do Vale, M. A. B.] Fed Univ Sao Joao Del Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadelli, M.; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gadfort, T.; Gibbard, B.; Gordon, H. A.; Hu, X.; Klimentov, A.; Kravchenko, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Metcalfe, J.; Nevski, P.; Okawa, H.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Park, W.; Pleier, M. -A.; Polychronakos, V.; Pravahan, R.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Snyder, S.; Steinberg, P.; Stumer, I.; Takai, H.; Tamsett, M. C.; Triplett, N.; Undrus, A.; Wenaus, T.; Ye, S.; Yu, D.; Zaytsev, A.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Badescu, E.; Boldea, V.; Buda, S. I.; Caprini, O.; Caprilli, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Cuciuc, C. -M.; Dinut, F.; Dita, P.; Dita, S.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. [Darlea, G. L.] Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Silva, M. L. Gonzalez; Otero y Garzon, G.; Piegaia, R.; Romeo, G.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Ask, S.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Buttinger, W.; Carter, J. R.; Chapman, J. D.; French, S. T.; Frost, J. A.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Moeller, V.; Mueller, T.; Parker, M. A.; Robinson, D.; Sandoval, T.; Thomson, M.; Ward, C. P.; Williams, S.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Koffas, T.; Lacey, J.; Marchand, J. F.; McCarthy, T. G.; Oakham, F. G.; Randrianarivony, K.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Anastopoulos, C.; Andari, N.; Anghinolfi, E.; Avolio, G.; Baak, M. A.; Banfi, D.; Battistin, M.; Bellomo, M.; Beltramello, O.; Berge, D.; Bogaerts, J. A.; Boyd, J.; Bremer, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Catmore, J. R.; Cattai, A.; Barajas, C. A. Chavez; Childers, J. T.; Chromek-Burckhart, D.; Cote, D.; Danielsson, H. O.; Dell'Acqua, A.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dopke, J.; Dovle, A. T.; Dudarev, A.; Duehrssen, M.; Ellis, N.; Elsing, M.; Fabre, C.; Facini, G.; Farthouat, P.; Fassnacht, P.; Franchino, S.; Francis, D.; Franz, S.; Froidevaux, D.; Gabaldon, C.; Garonne, V.; Gianotti, F.; Gillberg, D.; Godlewski, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Haas, S.; Hauschild, M.; Hawkings, R. J.; Heller, M.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Hubacek, Z.; Huhtinen, M.; Jaekel, M. R.; Jansen, H.; Jenni, P.; Jungst, R. M.; Kaneda, M.; Klioutchnikova, T.; Koeneke, K.; Lantzsch, K.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mapelli, L.; Martin, B.; Messina, A.; Meyer, J.; Michal, S.; Molfetas, A.; Morley, A. K.; Mornacchi, G.; Muenstermann, D.; Nairz, A. M.; Nakahama, Y.; Negri, G.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Ohm, C. C.; Pais, P.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Petersen, J.; Pommes, K.; Poppleton, A.; Poulard, G.; Prasad, S.; Raymond, M.; Rembser, C.; Dos Santos, D. Roda; Roe, S.; Salek, D.; Salzburger, A.; Savu, D. O.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Spiwoks, R.; Stewart, G. A.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van der Ster, D.; van Eldik, N.; Vandelli, W.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Winklmeier, F.; Wotschack, J.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Boveia, A.; Canelli, F.; Cheng, Y.; Choudalakis, G.; Fiascaris, M.; Gardner, R. W.; Jen-La Plante, I.; Kapliy, A.; Li, H. L.; Meehan, S.; Melachrinos, C.; Merritt, F. S.; Meyer, C.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Shochet, M. J.; Tompkins, L.; Tuggle, J. M.; Vukotic, I.; Webster', J. S.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Diaz, M. A.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Carquin, E.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lu, F.; Ouyang, Q.; Shan, L. Y.; Wang, J.; Xu, D.; Yao, L.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Han, L.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, K.; Liu, M.; Liu, Y.; Pais, P.; Peng, H.; Xu, C.; Xu, L.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Feng, C.; Ge, P.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Yang, H.] Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200030, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Clermont Univ, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] CNRS IN2P3, Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Chen, Y.; Dodd, J.; Guo, J.; Hu, D.; Hughes, E. W.; Nikiforou, N.; Parsons, J. A.; Penson, A.; Reale, V. Perez; Scherzer, M. I.; Spousta, M.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Williams, E.; Willis, W.; Wuif, E.; Zivkovic, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Boelaert, N.; Dam, M.; Gregersen, K.; Hansen, J. R.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Heisterkamp, S.; Jakobsen, S.; Joergensen, M. D.; Kadlecik, P.; Klinkby, E. B.; Loevschall-Jensen, A. E.; Lundquist, J.; Mackeprang, R.; Mehlhase, S.; Monk, J.; Petersen, T. C.; Pingel, A.; Simonyan, M.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, INFN Grp Colegato Cosenza, I-87036 Arcavacata Di Rende, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; Blocki, J.; de Renstrom, P. A. Bruckman; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Malecki, P.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Turala, M.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.; Zemla, A.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Cao, T.; Yagci, K. Dindar; Firan, A.; Hoffman, J.; Joffe, D.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Rios, R. R.; Sekula, S. J.; Stroynowski, R.; Wang, H.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Ahsan, M.; Izen, J. M.; Lou, X.; Namasivayam, H.; Reeves, K.; Wong, W. C.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Dassoulas, J. A.; Dietrich, J.; Ferrara, V.; Friedrich, C.; Glazov, A.; Goebel, M.; Fajardo, L. S. Gomes; Da Costa, J. Goncalves Pinto Firmino; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Hiller, K. H.; Huettmann, A.; Belenguer, M. Jimenez; Johnert, S.; Katzy, J.; Kono, T.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Cavalcanti, T. Perez; Peters, R. F. Y.; Petschull, D.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.; Zhu, H.] DESY, Hamburg, Germany. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Dassoulas, J. A.; Dietrich, J.; Ferrara, V.; Friedrich, C.; Glazov, A.; Goebel, M.; Fajardo, L. S. Gomes; Da Costa, J. Goncalves Pinto Firmino; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Hiller, K. H.; Huettmann, A.; Belenguer, M. Jimenez; Johnert, S.; Katzy, J.; Kono, T.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Cavalcanti, T. Perez; Peters, R. F. Y.; Petschull, D.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.; Zhu, H.] DESY, Zeuthen, Germany. [Bunse, M.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Reisinger, I.; Wittig, T.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Czodrowski, P.; Friedrich, F.; Grohs, J. P.; Kobel, M.; Leonhardt, K.; Mader, W. F.; Morgenstern, M.; Prudent, X.; Rudolph, C.; Schnoor, U.; Seifert, F.; Steinbach, P.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B.; Finelli, K. D.; Ko, B. R.; Kotwal, A.; Kruse, M. K.; Li, S.; Liu, M.; Oh, S. H.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Buckley, A. G.; Clark, P. J.; Debenedetti, C.; Walls, F. M. Garay; Harrington, R. D.; Korn, A.; Martin, V. J.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Schaelicke, A.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, R.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.; Volpi, G.] INFN Lab Nazl Frascati, Frascati, Italy. [Aad, G.; Ahles, F.; Amoroso, S.; Barber, T.; Bernhard, R.; Boehler, M.; Bnineliere, R.; Christov, A.; Consorti, V.; Fehling-Kaschek, M.; Flechl, M.; Giuliani, C.; Hartert, J.; Herten, G.; Jakobs, K.; Janus, M.; Kononov, A. I.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Lohwasser, K.; Ludwig, I.; Ludwig, J.; Madar, R.; Mahboubi, K.; Mohr, W.; Parzefall, U.; Rammensee, M.; Rave, T. C.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Siegert, F.; Stoerig, K.; Sundermann, J. E.; Temming, K. K.; Thoma, S.; Tsiskaridze, V.; Ungaro, F. C.; Venturi, M.; Vivarelli, I.; von Radziewslci, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Winkelmann, S.; Xie, S.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Abdelalim, A. A.; Alexandre, G.; Backes, M.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; Bucci, F.; Toro, R. Camacho; Clark, A.; Doglioni, C.; Ferrere, D.; Gadomslci, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Guescini, F.; Iacobucci, G.; La Rosa, A.; Latour, B. Martin Dit; Mermod, P.; Herrera, C. Mora; Nektarijevic, S.; Nessi, M.; Nikolics, K.; Pasztor, G.; Picazio, A.; Pohl, M.; Rosbach, K.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Beccherle, R.; Caso, C.; Darbo, G.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Univ Genoa, INFN Sez Genova, Genoa, Italy. [Barberis, D.; Caso, C.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Tskhadadaze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Khubuab, J.; Mchedlidze, G.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Bussey, P.; Buttar, C. M.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Dovle, A. T.; Edwards, N. C.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Kar, D.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Quilty, D.; Ravenscroft, T.; Robson, A.; Saxon, D. H.; Smith, K. M.; Denis, R. D. St.; Steele, G.; Thompson, A. S.; Wraight, K.; Wright, M.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bierwagen, K.; Blumenschein, U.; Brandt, O.; Evangelakou, D.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Hensel, C.; Kawamura, G.; Keil, M.; Knue, A.; Kohn, F.; Krieger, N.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Meyer, J.; Morel, J.; Nackenhorst, .; Pashapour, S.; Peters, R. F. Y.; Quadt, A.; Roe, A.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Schroeder, T. Vazquez; Weingarten, J.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] Univ Grenoble 1, Lab Phys Subatom & Cosmologie, Grenoble, France. [Albrand, S.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] CNRS IN2P3, Grenoble, France. [Albrand, S.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] Inst Natl Polytech Grenoble, F-38031 Grenoble, France. [Addy, T. N.; Harvey, A.; McFarlane, K. W.; Shin, T.; Vassilakopoulos, Vi.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Belloni, A.; Butler, B.; Catastini, R.; Conti, G.; Franklin, M.; Huth, J.; Jeanty, L.; Mateos, D. Lopez; Mercurio, K. M.; Mills, C.; Morii, M.; Skottowe, H. P.; Yen, A. L.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Anders, G.; Andrei, V.; Davygora, Y.; Dietzsch, T. A.; Dunford, M.; Hanke, P.; Henke, M.; Hofmann, J. I.; Khomich, A.; Kluge, E. -E.; Laier, H.; Lang, V. S.; Lendermann, V.; Lepold, F.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Kasieczka, G.; Narayan, R.; Schaetzeb, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Kugel, A.; Schroer, N.] Heidelberg Univ, ZITI Inst Tech lnformat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Evans, H.; Gagnon, P.; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Price, D.; Whittington, D.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jussel, P.; Kneringer, E.; Ritsch, E.] Leopold Franzens Univ, Inst Astro & Teilchenphy, Innsbruck, Austria. [Cinca, D.; Gandrajula, R. P.; Halladjian, G.; Limper, M.; Mallik, U.; Mandrysch, R.; Morange, N.; Pylypchenko, Y.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Ruiz-Martinez, A.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Aleksandrov, I. N.; Bardin, D. Y.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Grigalashvili, N.; Huseynov, N.; Kazarinov, M. Y.; Kharchenko, D.; Ithramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Potraptm, I. N.; Pozdnyakov, V.; Rumyantsev, L.; Rusakovich, N. A.; Sadykov, R.; Shiyakova, M.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.; Zimin, N. I.] Joint Inst Nucl Res Dubna, Dubna, Russia. [Amako, K.; Arai, Y.; Doi, Y.; Haruyama, T.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Zaki, J. Ka; Kohriki, T.; Kondo, T.; Makida, Y.; Mitsui, S.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Hayakawa, T.; King, M.; Kishimoto, T.; Kitamura, T.; Kurashige, H.; Matsushita, T.; Ochi, A.; Suzuki, Y.; Takeda, H.; Tani, K.; Watanabe, I.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Sasao, N.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Consejo Nacl Invest Cient & Tecn, La Plata, Argentina. [Allison, L. J.; Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Bianco, M.; Cataldi, G.; Chiodini, G.; Gorini, E.; Grancagnolo, F.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Univ Salerno, INFN Sez Lecce, Lecce, Italy. [Bianco, M.; Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salerno, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Greenshaw, T.; Gwilliam, C. B.; Hayward, H. S.; Jackson, J. N.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Schnellbach, Y. J.; Sellers, G.; Vossebeld, J. H.; Waller, P.; Wrona, B.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia. [Bona, M.; Carter, A. A.; Cerrito, L.; Eisenhandler, E.; Ellis, K.; Fletcher, G.; Goddard, J. R.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Rizvi, E.; Salamanna, G.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Alam, M. A.; Berry, T.; Boisvert, V.; Brooks, T.; Cantrill, R.; Cooper-Smith, N. J.; Cowan, G.; Duguid, L.; Edwards, C. A.; George, S.; Gibson, S. M.; Goncalo, R.; Hayden, D.; Vazquez, J. G. Panduro; Pastore, Fr.; Rose, M.; Spano, F.; Strong, J. A.; Teixeira-Dias, P.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Baker, S.; Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Chislett, R. T.; Christidi, I. A.; Cooper, B. D.; Davison, A. R.; Dobson, E.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Lambourne, L.; Nash, M.; Nurse, E.; Ochoa, M. I.; Pilkington, A. D.; Prabhu, R.; Sherwood, P.; Simmons, B.; Taylor, C.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Bernius, C.; Dhullipudi, R.; Greenwood, Z. D.; Sawyer, L.; Sircar, A.; Subramaniam, R.; Tamsett, M. C.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, .; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Range-Smith, C.; Ridel, M.; Roos, L.; Torres, H.; Trincaz-Duvold, S.; Vannucci, F.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, .; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Range-Smith, C.; Ridel, M.; Roos, L.; Torres, H.; Trincaz-Duvold, S.; Vannucci, F.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, .; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Range-Smith, C.; Ridel, M.; Roos, L.; Torres, H.; Trincaz-Duvold, S.; Vannucci, F.] CNRS IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Jarlskog, G.; Lytken, E.; Meirose, B.; Mjornmark, J. U.; Smirnova, O.; Wielers, M.] Lund Univ, Inst Fys, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Labarga, L.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Arnaez, O.; Blum, W.; Buescher, V.; Caputo, R.; Eckweiler, S.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Coeringer, C.; Handel, C.; Heck, T.; Hohlfeld, M.; Hsu, P. J.; Huelsing, T. A.; Ji, W.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lungwitz, M.; Masetti, L.; Meyer, C.; Moreno, D.; Moritz, S.; Mueller, T.; Neusiedl, A.; Poettgen, R.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Almond, J.; Born, M.; Brown, G.; Chavda, V.; Cox, B. E.; Da Via, C.; Forti, A.; Howarth, J.; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Marx, M.; Masik, J.; Messina, A.; Neep, T. J.; Oh, A.; Owen, M.; Pais, P.; Pater, J. R.; Robinson, J. E. M.; Tomlinson, L.; Watts, S.; Woudstra, M. J.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Barber, M.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Dovle, A. T.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Messina, A.; Monnier, E.; Nagai, Y.; Odier, J.; Pais, P.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Barber, M.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Ertel, E.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Nagai, Y.; Odier, J.; Pais, P.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] CNRS IN2P3, Marseille, France. [Brau, B.; Colon, G.; Dallapiccola, C.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Dufour, M-A.; Klemetti, M.; Mantifel, R.; Pais, P.; Robertson, S. H.; Schram, M.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Diglio, S.; Hamano, K.; Jennens, D.; Kubota, T.; Limosani, A.; Hanninger, G. Nunes; Phan, A.; Shao, Q. T.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Volpi, M.; White, M. J.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Armbruster, A. J.; Chapman, J. W.; Cirilli, M.; Dai, T.; Diehl, E. B.; Dubbert, J.; Feng, H.; Ferretti, C.; Goldfarb, S.; Harper, D.; Levin, D.; Li, X.; Liu, L.; Mc Kee, S. P.; Neal, H. A.; Pais, P.; Panikashvili, N.; Qian, J.; Scheirich, D.; Searcy, J.; Thun, R. P.; Walch, S.; Wilson, A.; Wooden, G.; Wu, Y.; Xu, L.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Ge, P.; Hauser, R.; Holzbauer, J. L.; Huston, J.; Koll, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schwienhorst, R.; Stelzer, H. J.; Tollefson, K.; True, P.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI USA. [Alessandria, F.; Alimonti, G.; Andreazza, A.; Besana, M. I.; Broggi, F.; Carminati, L.; Cavalli, D.; Citterio, M.; Consonni, S. M.; Costa, G.; Fanti, M.; Favareto, A.; Giugni, D.; Koletsou, I.; Lari, T.; Mandelli, L.; Mazzanti, M.; Meloni, F.; Meroni, C.; Pais, P.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Rivoltella, G.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Volpini, G.] Univ Milan, INFN Sez Milano, Milan, Italy. [Andreazza, A.; Besana, M. I.; Carminati, L.; Consonni, S. M.; Fanti, M.; Favareto, A.; Meloni, F.; Perini, L.; Pizio, C.; Ragusa, F.; Rivoltella, G.; Simoniello, R.; Turra, R.] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Satsounkevitch, I.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus. [Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Asbah, N.; Azuelos, G.; Banerjee, P.; Bouchami, J.; Dallaire, F.; Davies, M.; Gauthier, L.; Giunta, M.; Leroy, C.; Martin, J. P.; Rezvani, R.; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.] Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] ITEP, Moscow, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.] Moscow Engn & Phys Inst MEPhI, Moscow, Russia. [Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Beale, S.; Becker, S.; Biebel, O.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; de Graat, J.; Duckeck, G.; Ebke, J.; Elmsheuser, J.; Engl, A.; Galea, C.; Heller, C.; Hertenberger, R.; Legger, F.; Lorenz, J.; Mann, A.; Meineck, C.; Nunnemann, T.; Oakes, L. B.; Rauscher, F.; Reznicek, P.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Schieck, J.; Schmitt, C.; Staude, A.; Vladoiu, D.; Walker, R.; Will, J. Z.; Wittkowslci, J.; Zibell, A.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bittner, B.; Bronner, J.; Capriotti, D.; Compostella, G.; Cortiana, G.; Flowerdew, M. J.; Giovannini, P.; Goblirsch-Kolb, M.; Ince, T.; Jantsch, A.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kotov, S.; Kroha, H.; Macchiolo, A.; Manfredini, A.; Menke, S.; Moser, H. G.; Nagel, M.; Nisius, R.; Oberlack, H.; Pahl, C.; Too, G. E. Pospelov; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Stern, S.; Stonjek, S.; Vanadia, M.; von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Shimizu, S.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Shimizu, S.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; della Volpe, D.; Di Donato, C.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Patricelli, S.; Sanchez, A.; Sekhniaidze, G.] Univ Naples Federico II, INFN Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Chiefari, G.; della Volpe, D.; Di Donato, C.; Giordano, R.; Merola, L.; Patricelli, S.; Sanchez, A.] Univ Naples Federico II, Dipartimento Sci Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Chelstowska, M. A.; Dao, V.; De Groot, N.; Filthaut, F.; Klok, P. F.; Koetsveld, F.; Konig, A. C.; Raas, M.; Salvucci, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Messina, A.; Mussche, I.; Ottersbach, J. P.; Pais, P.; Pani, P.; Ruckstuhl, N.; Ta, D.; Tsiakiris, M.; Valencic, N.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; Van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Pani, P.; Ruckstuhl, N.; Ta, D.; Tsiakiris, M.; Valencic, N.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; Van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.] Univ Amsterdam, Amsterdam, Netherlands. [Calkins, R.; Chakraborty, D.; Cole, S.; de Lima, J. G. Rocha; Suhr, C.; Yurkewicz, A.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL USA. [Anisenkov, A. V.; Beloborodova, O. L.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Skovpen, K. Yu.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Budick, B.; Casadei, D.; Cranmer, K.; Haas, A.; van Huysduynen, L. Hooft; Kaplan, B.; Konoplich, R.; Krasznahorkay, A.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.; Prokofiev, K.] NYU, Dept Phys, New York, NY 10003 USA. [Fisher, M. J.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Strang, M.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Gutierrez, P.; Jana, D. K.; Marzin, A.; Meera-Lebbai, R.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Snow, J.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Khanov, A.; Rizatdinova, F.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Hamal, P.; Hrabovslcy, M.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Brost, E.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Reinsch, A.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Auge, E.; Binet, S.; Bourdarios, C.; De la Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grimm, J. -F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Niedercorn, F.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Teinturier, M.; Tran, H. L.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Auge, E.; Binet, S.; Bourdarios, C.; De la Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grimm, J. -F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Niedercorn, F.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Teinturier, M.; Tran, H. L.; Zerwas, D.; Zhang, Z.] CNRS IN2P3, Orsay, France. [Hanagaki, K.; Hirose, M.; Lee, J. S. H.; Meguro, T.; Nomachi, M.; Okamura, W.; Sugaya, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Buran, T.; Cameron, D.; Gjelsten, B. K.; Gramstad, E.; Lund, E.; Ould-Saada, F.; Pais, P.; Pajchel, K.; Pedersen, M.; Read, A. L.; Rohne, O.; Smestad, L.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Apolle, R.; Barr, A. J.; Boddy, C. R.; Buchanan, J.; Buckingham, R. M.; Cooper-Sarkar, A. M.; Dafinca, A.; Davies, E.; Gallas, E. J.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; King, R. S. B.; Kogan, L. A.; Larner, A.; Lewis, A.; Liang, Z.; Livermore, S. S. A.; Mattravers, C.; Nickerson, R. B.; Pachal, K.; Pais, P.; Pinder, A.; Robichaud-Veronneau, A.; Ryder, N. C.; Sawyer, C.; Short, D.; Tseng, J. C-L.; Vickey, T.; Viehhauser, G. H. A.; Weidberg, A. R.; Whitehead, S. R.; Young, C. J. S.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Colombo, T.; Conta, C.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Univ Pavia, INFN Sez Pavia, I-27100 Pavia, Italy. [Colombo, T.; Conta, C.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Degenhardt, J.; Fratina, S.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Keener, P. T.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Marshall, Z.; Newcomer, F. M.; Olivito, D.; Ospanov, R.; Pais, P.; Reece, R.; Saxon, J.; Schaefer, D.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Van Berg, R.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Bertolucci, F.; Cascella, M.; Cavasinni, V.; Del Prete, T.; Giannetti, R.; Roda, C.; Sarri, F.; White, S.; Zinonos, Z.] Univ Pisa, INFN Sez Pisa, Pisa, Italy. [Bertolucci, F.; Cascella, M.; Cavasinni, V.; Del Prete, T.; Dotti, A.; Giannetti, R.; Roda, C.; Sarri, F.; White, S.; Zinonos, Z.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Escobar, C.; Kittelmann, T.; Mueller, J.; Prieur, D.; Sapp, K.; Savinov, V.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Dos Santo, S. P. Amor; Amorim, A.; Anjos, N.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Wemans, A. Do Valle; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Jorge, P. M.; Lopes, L.; Machado Miguens, J.; Maio, A.; Maneira, J.; Marques, C. N.; Oliveira, M.; Onofre, A.; Pais, P.; Palma, A.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Tamsett, M. C.; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. [Bohm, J.; Chudoba, J.; Denisov, S. P.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Messina, A.; Mikestikova, M.; Myska, M.; Nemecek, S.; Pais, P.; Ruzicka, P.; Schovancova, J.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Tic, T.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Gallus, P.; Gunther, J.; Jakubek, J.; Kohout, Z.; Kral, V.; Pospisil, S.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solar, M.; Solc, J.; Sopko, V.; Sopko, B.; Stekl, I.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, Prague, Czech Republic. [Balek, P.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Torregrosa, E. Fullana; Kodys, P.; Leitner, R.; Novakova, J.; Pleskot, V.; Rybar, M.; Spousta, M.; Sykora, T.; Tas, P.; Valkar, S.; Vorobel, V.; Wilhelm, I.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Ammosov, V. V.; Borisov, A.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Ivashin, A. V.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Pais, P.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, .; Zmouchko, V. V.] Inst High Energy Phys, State Res Ctr Inst, Protvino, Russia. [Adye, T.; Apolle, R.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Gillman, A. R.; Haywood, S. J.; Kirk, J.; Mattravers, C.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Nash, M.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Ruthetford Appleton Lab, Particle Phys Dept, Didcot, Oxon, England. [Benslama, K.] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Artoni, G.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Pedis, D.; De Salvo, A.; De Zorzi, G.; Dionisi, C.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Rossi, E.; Tehrani, F. Safai; Sidoti, A.; Camillocci, E. Solfaroli; Vari, R.; Veneziano, S.; Zanello, L.] Univ Roma La Sapienza, INFN Sez Roma 1, I-00185 Rome, Italy. [Artoni, G.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Zorzi, G.; Dionisi, C.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Messina, A.; Rossi, E.; Camillocci, E. Solfaroli; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Di Simone, A.; Liberti, B.; Marchese, F.; Mazzaferro, L.; Salamon, A.; Santonico, R.] Univ Roma Tor Vergata, INFN Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Di Simone, A.; Liberti, B.; Marchese, F.; Mazzaferro, L.; Salamon, A.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Branchini, P.; Ceradini, F.; Di Luise, S.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Stanescu, C.; Trovatelli, M.] Univ Roma Tre, INFN Sez Roma Tre, Rome, Italy. [Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Luise, S.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.; Lablak, S.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA Marrakech, Fac Sci Semlatia, Ayyad, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Abreu, H.; Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Bolnet, N. M.; Boonekamp, M.; Chevalier, L.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Guyot, C.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Legendre, M.; Maiani, C.; Mal, P.; Ramos, J. A. Manjarres; Mansoulie, B.; Martinez, H.; Meric, N.; Meyer, J-P.; Mijovic, L.; Mountricha, E.; Hong, V. Nguyen Thi; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Resende, B.; Royon, C. R.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.; Tsionou, D.; Vranjes, N.; Xia, M.; Xu, C.] Lois Fimdament Univ, Inst Rech, DSM IRFU, CEA Saclay,Commissariat Energie Atom & Energies A, Gif Sur Yvette, France. [Damiani, D. S.; Grillo, A. A.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Mitrevski, J.; Nielsen, J.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Becicingham, M.; Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Hsu, S. -C.; Keller, J. S.; Lubatti, H. J.; Rompotis, N.; Rothberg, J.; Verducci, M.; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Mcfayden, J. A.; Miyagawa, P. S.; Owen, S.; Paganis, E.; Suruliz, K.; Tovey, D. R.; Tua, A.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Ibragimov, I.; Ikematsu, K.; Rammes, M.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Dawe, E.; Godfrey, J.; Kvita, J.; O'Neil, D. C.; Petteni, M.; Stelzer, B.; Tanasijczuk, A. J.; Trottier-McDonald, M.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Mayes, J. Backus; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Hansson, P.; Kagan, M.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nelson, T. K.; Piacquadio, G.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Strauss, E.; Su, D.; Swiatlowski, M.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Batkova, L.; Blazek, T.; Federic, P.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bnincko, D.; Ferencei, J.; Kladiva, E.; Seman, M.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnuclear Phys, Kosice 04353, Slovakia. [Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Carrillo-Montoya, G. D.; Leney, K. J. C.; Garcia, B. R. Mellado; Ruan, X.; Boeriu, . E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Asman, B.; Bendtz, K.; Bohm, C.; Clement, C.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Holmgren, S. O.; Johansen, M.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Papadelis, A.; Petridis, A.; Plucinski, P.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Asman, B.; Bendtz, K.; Clement, C.; Gellerstedt, K.; Hellman, S.; Johansen, M.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Petridis, A.; Plucinski, P.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Ahmad, A.; Arfaoui, S.; DeWilde, B.; Engelmann, R.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Puldon, D.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Ahmad, A.; Arfaoui, S.; DeWilde, B.; Engelmann, R.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Puldon, D.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Bartsch, V.; De Santo, A.; Martin-Haugh, S.; Potter, C. J.; Rose, A.; Salvatore, F.; Castillo, I. Santy; Sutton, M. R.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Bangert, A.; Black, C. W.; Cuthbert, C.; Jeng, G. -Y.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Waugh, A. T.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Chu, M. L.; Hou, S.; Jamin, D. O.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, D.; Mazini, R.; Ren, Z. L.; Soh, D. A.; Teng, P. K.; Wang, J.; Wang, S. M.; Weng, Z.; Zhang, L.; Zhou, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Di Mattia, A.; Kajomovitz, E.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; Vallecorsa, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Bella, G.; Benary, O.; Benhammou, Y.; Etzion, E.; Gershon, A.; Gueta, O.; Guttman, N.; Munwes, Y.; Oren, Y.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astronomy, IL-69978 Tel Aviv, Israel. [Bachas, K.; Glcialas, I.; Iliadis, D.; Kordas, K.; Kouskoura, V.; Nomidis, I.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yamazaki, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yamazaki, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Ishitsuka, M.; Jinnouchi, O.; Kanno, T.; Kuze, M.; Nagai, R.; Nobe, T.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Bailey, D. C.; Brelier, B.; Cheung, S. L.; Farooque, T.; Fatholahzadeh, B.; Gibson, A.; Ilic, N.; Keung, J.; Krieger, P.; Orr, R. S.; Polifka, R.; Rosenbaum, G. A.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Spreitzer, T.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Fortin, D.; Gingrich, D. M.; Koutsman, A.; Losty, M. J.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Bustos, A. C. Florez; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hanawa, K.; Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Kurata, M.; Nagai, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Napier, A.; Rolli, S.; Sliwa, K.; Todorova-Nova, S.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Loureiro, K. F.; Mendoza Navas, L.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Farrell, S.; Gerbaudo, D.; Eschrich, I. Gough; Lankford, A. J.; Magnoni, L.; Mete, A. S.; Nelson, A.; Rao, K.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Taffard, A.; Toggerson, B.; Unel, G.; Werth, M.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Pinamonti, M.; Shaw, K.; Soualah, R.] INFN Grp Collegaw Udine, Udine, Italy. [Acharya, B. S.; Soualah, R.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Shaw, K.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Coggeshall, J.; Cortes-Gonzalez, A.; Errede, D.; Errede, S.; Lie, K.; Liss, T. M.; McCarn, A.; Neubauer, M. S.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Brenner, R.; Buszello, O.; Coniavitis, E.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Pelikan, D.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladoid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Rsica Corpuscular IFIC, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladoid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladoid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladoid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Ist Microelect Barcelona IMB CNM, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Torro Pastor, E.; Valero, A.; Valladoid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] CSIC, Valencia, Spain. [Axen, D.; Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Loh, C. W.; Mills, W. J.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Astbury, A.; Bansal, V.; Berghaus, F.; Bernlochner, F. U.; Courneyea, L.; Fincke-Keeler, M.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Lessard, J-R.; Mariono, C. P.; Martyniuk, A. C.; McPharson, R. A.; Ouellette, E. 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[Fleischmann, P.; Redelbach, A.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Barisonzi, M.; Becker, K.; Becks, K. H.; Beermann, T. A.; Boek, J.; Boek, T. T.; Braun, H. M.; Cornelissen, T.; Duda, D.; Fischer, J.; Fleischmann, S.; Flick, T.; Gorfine, G.; Hamacher, K.; Harenberg, T.; Hirschbuehl, D.; Kalinin, S.; Kersten, S.; Khoroshilov, A.; Kohlmann, S.; Lenzen, G.; Maettig, P.; Mechtel, M.; Neumann, M.; Pataraia, S.; Sandhoff, M.; Sartisohn, G.; Sturm, P.; Wagner, W.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich C Phys, Wuppertal, Germany. [Adelman, J.; Baker, O. K.; Bedikian, S.; Almenar, C. Cuenca; Cummings, J.; Czyczula, Z.; Demers, S.; Erdmann, J.; Garberson, F.; Golling, T.; Guest, D.; Henrichs, A.; Lagouri, T.; Lee, L.; Leister, A. G.; Loginov, A.; Tipton, P.; Wall, R.; Walsh, B.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.; Wicke, D.] Inst Natl Phys Nucl & Phys Particules IN2P3, Ctr Calcul, Villeurbantze, France. [Acharya, B. S.; Tamsett, M. C.] Kings Coll London, Dept Phys, London, England. [Amorim, A.; Gomes, A.; Maio, A.; Pina, J.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amorim, A.; Gomes, A.; Maio, A.; Pina, J.] Univ Lisbon, CFNUL, P-1699 Lisbon, Portugal. [Bawa, H. S.; Gao, Y. S.; Lowe, A. J.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beloborodova, O. L.; Maximov, D. A.; Talyshev, A. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Carvalho, J.; Fiolhais, M. C. N.; Oliveira, M.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Demirkoz, B.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Dhullipudi, R.; Greenwood, Z. D.; Sawyer, L.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Wemans, A. Do Valle] Univ Nova Lisboa, Dept Fis, Fac Ciencias & Tecnol, Caparica, Portugal. [Wemans, A. Do Valle] Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, Caparica, Portugal. [Glcialas, I.; Papageorgiou, K.] Univ Aegean, Dept Financial & Management Engn, Chios, Greece. [Grinstein, S.; Juste Rozas, A.; Martinez, M.] ICREA, Barcelona, Spain. [Huseynov, N.] Azerbaijan Acad Sci, Inst Phys, Baku 370143, Azerbaijan. [Kono, T.; Wildt, M. A.] Univ Hamburg, Inst Expt Phys, Hamburg, Germany. [Dhullipudi, R.; Greenwood, Z. D.; Sawyer, L.] Manhattan Coll, New York, NY USA. [Liang, Z.; Soh, D. A.; Weng, Z.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou, Peoples R China. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Mal, P.] Natl Inst Sci Educ & Res, Sch Phys Sci, Bhubaneswar, Orissa, India. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys, Dolgoprudnyi, Russia. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Technol State Univ, Dolgoprudnyi, Russia. 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RI Ferrando, James/A-9192-2012; Boyko, Igor/J-3659-2013; Brooks, William/C-8636-2013; Tudorache, Alexandra/L-3557-2013; Tudorache, Valentina/D-2743-2012; Moraes, Arthur/F-6478-2010; Gabrielli, Alessandro/H-4931-2012; Marti-Garcia, Salvador/F-3085-2011; Shabalina, Elizaveta/M-2227-2013; Wolters, Helmut/M-4154-2013; Snesarev, Andrey/H-5090-2013; Warburton, Andreas/N-8028-2013; Jakoubek, Tomas/G-8644-2014; Staroba, Pavel/G-8850-2014; Kupco, Alexander/G-9713-2014; de Groot, Nicolo/A-2675-2009; Hejbal, Jiri/H-1358-2014; Marcisovsky, Michal/H-1533-2014; Mikestikova, Marcela/H-1996-2014; Lysak, Roman/H-2995-2014; Tomasek, Lukas/G-6370-2014; Svatos, Michal/G-8437-2014; Chudoba, Jiri/G-7737-2014; Peleganchuk, Sergey/J-6722-2014; Bosman, Martine/J-9917-2014; Sukharev, Andrey/A-6470-2014; Solfaroli Camillocci, Elena/J-1596-2012; Lee, Jason/B-9701-2014; Kuday, Sinan/C-8528-2014; Smirnova, Oxana/A-4401-2013; Zimmermann, Claus/E-9598-2014; Fabbri, Laura/H-3442-2012; Villa, Mauro/C-9883-2009; Carvalho, Joao/M-4060-2013; Nozka, Libor/G-5550-2014; Nemecek, Stanislav/G-5931-2014; Kepka, Oldrich/G-6375-2014; Lokajicek, Milos/G-7800-2014; Castro, Nuno/D-5260-2011; Grinstein, Sebastian/N-3988-2014; Wemans, Andre/A-6738-2012; Gutierrez, Phillip/C-1161-2011; Ventura, Andrea/A-9544-2015; Livan, Michele/D-7531-2012; De, Kaushik/N-1953-2013; Mitsou, Vasiliki/D-1967-2009; Joergensen, Morten/E-6847-2015; Riu, Imma/L-7385-2014; Cabrera Urban, Susana/H-1376-2015; Mir, Lluisa-Maria/G-7212-2015; Della Pietra, Massimo/J-5008-2012; Cavalli-Sforza, Matteo/H-7102-2015; Petrucci, Fabrizio/G-8348-2012; Negrini, Matteo/C-8906-2014; Ferrer, Antonio/H-2942-2015; Hansen, John/B-9058-2015; Grancagnolo, Sergio/J-3957-2015; spagnolo, stefania/A-6359-2012; Ciubancan, Liviu Mihai/L-2412-2015; Shmeleva, Alevtina/M-6199-2015; Camarri, Paolo/M-7979-2015; Gavrilenko, Igor/M-8260-2015; Akimov, Andrey/N-1769-2015; Tikhomirov, Vladimir/M-6194-2015; Chekulaev, Sergey/O-1145-2015; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; Andreazza, Attilio/E-5642-2011; Demirkoz, Bilge/C-8179-2014; Mashinistov, Ruslan/M-8356-2015; Buttar, Craig/D-3706-2011; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Pacheco Pages, Andres/C-5353-2011; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Olshevskiy, Alexander/I-1580-2016; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Mora Herrera, Maria Clemencia/L-3893-2016; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; KHODINOV, ALEKSANDR/D-6269-2015; Goncalo, Ricardo/M-3153-2016; Gauzzi, Paolo/D-2615-2009; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Monzani, Simone/D-6328-2017; Grancagnolo, Francesco/K-2857-2015; Korol, Aleksandr/A-6244-2014; Karyukhin, Andrey/J-3904-2014; Capua, Marcella/A-8549-2015; Tartarelli, Giuseppe Francesco/A-5629-2016; Fassi, Farida/F-3571-2016; la rotonda, laura/B-4028-2016; 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Fassi, Farida/0000-0002-6423-7213; la rotonda, laura/0000-0002-6780-5829; Osculati, Bianca Maria/0000-0002-7246-060X; Amorim, Antonio/0000-0003-0638-2321; Santos, Helena/0000-0003-1710-9291; Coccaro, Andrea/0000-0003-2368-4559; Casadei, Diego/0000-0002-3343-3529; Della Volpe, Domenico/0000-0001-8530-7447; Mendes Saraiva, Joao Gentil/0000-0002-7006-0864; Pina, Joao /0000-0001-8959-5044; Salamanna, Giuseppe/0000-0002-0861-0052; Veneziano, Stefano/0000-0002-2598-2659; Lacasta, Carlos/0000-0002-2623-6252; Price, Darren/0000-0003-2750-9977; Belanger-Champagne, Camille/0000-0003-2368-2617 FU NPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union; ERC, European Union; NSRF, European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; ISF, Israel; MINERVA, Israel; GIF, Israel; DIP, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; GRICES, Portugal; FCT, Portugal; MERYS (MECTS), Romania; MES of Russia, Russian Federation; ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America FX We acknowledge the support of NPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; ISF, MINERVA, GIF, DIP and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW, Poland; GRICES and FCT, Portugal; MERYS (MECTS), Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. NR 41 TC 18 Z9 18 U1 7 U2 215 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0550-3213 EI 1873-1562 J9 NUCL PHYS B JI Nucl. Phys. B PD OCT 21 PY 2013 VL 875 IS 3 BP 483 EP 535 DI 10.1016/j.nuclphysb.2013.07.025 PG 53 WC Physics, Particles & Fields SC Physics GA 220QJ UT WOS:000324601700001 ER PT J AU Bacchetta, A Prokudin, A AF Bacchetta, Alessandro Prokudin, Alexei TI Evolution of the helicity and transversity. Transverse-momentum-dependent parton distributions SO NUCLEAR PHYSICS B LA English DT Article ID TO-LEADING ORDER; DEEP-INELASTIC SCATTERING; FINAL-STATE INTERACTIONS; DRELL-YAN; SPIN ASYMMETRIES; BOSON PRODUCTION; QCD; LEPTOPRODUCTION; RESUMMATION; COLLISIONS AB We examine the QCD evolution of the helicity and transversity parton distribution functions when including also their dependence on transverse momentum. Using an appropriate definition of these polarized transverse momentum distributions (TMDs), we describe their dependence on the factorization scale and rapidity cutoff, which is essential for phenomenological applications. (C) 2013 Elsevier B.V. All rights reserved. C1 [Bacchetta, Alessandro] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Bacchetta, Alessandro] INFN Sez Pavia, I-27100 Pavia, Italy. [Prokudin, Alexei] Jefferson Lab, Newport News, VA 23606 USA. RP Prokudin, A (reprint author), Jefferson Lab, 12000 Jefferson Ave, Newport News, VA 23606 USA. EM alessandro.bacchetta@unipv.it; prokudin@jlab.org RI Bacchetta, Alessandro/F-3199-2012 OI Bacchetta, Alessandro/0000-0002-8824-8355 FU US DOE [DE-AC05-06OR23177]; Italian MIUR [PRIN 2008EKLACK]; European Community [283286] FX We would like to thank Ted Rogers for multiple discussions, help, and encouragement during preparation of this paper. We thank John Collins for useful discussions and Alberto Accardi for careful reading of the manuscript. Authored by a Jefferson Science Associate, LLC, under US DOE Contract No. DE-AC05-06OR23177. A. Bacchetta is partially supported by the Italian MIUR through the PRIN 2008EKLACK, and by the European Community through the Research Infrastructure Integrating Activity "HadronPhysics3" (Grant Agreement No. 283286) under the 7th Framework Programme. NR 61 TC 20 Z9 20 U1 0 U2 1 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0550-3213 J9 NUCL PHYS B JI Nucl. Phys. B PD OCT 21 PY 2013 VL 875 IS 3 BP 536 EP 551 DI 10.1016/j.nuclphysb.2013.07.013 PG 16 WC Physics, Particles & Fields SC Physics GA 220QJ UT WOS:000324601700002 ER PT J AU Moriya, K Leckey, JP Shepherd, MR Bauer, K Bennett, D Egiyan, H Frye, J Gonzalez, J Henderson, SJ Lawrence, D Mitchell, R Smith, ES Smith, P Somov, A AF Moriya, K. Leckey, J. P. Shepherd, M. R. Bauer, K. Bennett, D. Egiyan, H. Frye, J. Gonzalez, J. Henderson, S. J. Lawrence, D. Mitchell, R. Smith, E. S. Smith, P. Somov, A. TI A measurement of the energy and timing resolution of the GlueX Forward Calorimeter using an electron beam SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE GlueX; Jefferson Lab; Calorimetry; Lead glass; Flash ADC ID TAGGED PHOTON-BEAM AB The performance of the GlueX Forward Calorimeter was studied using a small version of the detector and a variable energy electron beam derived from the Hall B tagger at Jefferson Lab. For electron energies from 110 MeV to 260 MeV, which are near the lower-limits of the design sensitivity, the fractional energy resolution was measured to range from 20% to 14%, which meets the design goals. The use of custom 250 MHz flash ADCs for readout allowed precise measurements of signal arrival times. The detector achieved timing resolutions of 0.38 ns for a single 100 mV pulse, which will allow timing discrimination of photon beam bunches and out-of-time background during the operation of the GlueX detector. (c) 2013 Elsevier B.V. All rights reserved. C1 [Moriya, K.; Leckey, J. P.; Shepherd, M. R.; Bauer, K.; Bennett, D.; Frye, J.; Henderson, S. J.; Mitchell, R.; Smith, P.] Indiana Univ, Bloomington, IN 47405 USA. [Egiyan, H.; Gonzalez, J.; Lawrence, D.; Smith, E. S.; Somov, A.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. RP Shepherd, MR (reprint author), Indiana Univ, Bloomington, IN 47405 USA. EM mashephe@indiana.edu FU Department of Energy [DE-FG02-05ER41374]; United States Department of Energy [DE-AC05-06OR23177] FX We would like to thank the CLAS Collaboration and the members of the HD-ICE experiment, for their hospitality, time and effort, which made our beam test possible. We would especially like to thank Eugene Pasyuk and Sergey Boyarinov for their help. This work was supported by the Department of Energy under contract DE-FG02-05ER41374. Jefferson Science Associates, LLC operated Thomas Jefferson National Accelerator Facility for the United States Department of Energy under contract DE-AC05-06OR23177. NR 10 TC 3 Z9 3 U1 1 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD OCT 21 PY 2013 VL 726 BP 60 EP 66 DI 10.1016/j.nima.2013.05.109 PG 7 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 206WU UT WOS:000323557200009 ER PT J AU Wang, ZH Morris, CL AF Wang, Zhehui Morris, Christopher L. TI Tracking fast neutrons SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Fast neutron tracking; Ion tracking; Light field imaging ID TIME PROJECTION CHAMBER; DETECTORS; ELECTRONS AB Both neutron absorption and elastic scattering can be used to measure neutron momentum. Based on elastic collisions, the linear momentum of a fast neutron can be measured from as few as two consecutive recoil ion tracks plus the vertex position of the third collision, or two and half ion tracks. If the time delay between the first two consecutive ion tracks is also measured, the number of ion tracks can be reduced to one and a half. The angular and magnitude resolutions are limited by ion range straggling to about 10%. Multi-wire proportional chambers and light-field imaging can be used for fast neutron tracking. Light-field imaging is free of charge-diffusion-induced image blur, but the limited number of photons available can be a challenge. H-1, H-2 and He-3 could be used for the initial development of fast neutron trackers based on light-field imaging. (C) 2013 Elsevier B.V. All rights reserved. C1 [Wang, Zhehui; Morris, Christopher L.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Wang, ZH (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM zwang@lanl.gov OI Morris, Christopher/0000-0003-2141-0255 NR 40 TC 0 Z9 0 U1 0 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD OCT 21 PY 2013 VL 726 BP 145 EP 154 DI 10.1016/j.nima.2013.05.167 PG 10 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 206WU UT WOS:000323557200021 ER PT J AU Lees, JP Poireau, V Tisserand, V Grauges, E Palano, A Eigen, G Stugu, B Brown, DN Kerth, L Kolomensky, YG Lynch, G Koch, H Schroeder, T Asgeirsson, DJ Hearty, C Mattison, TS McKenna, JA So, RY Khan, A Blinov, VE Buzykaev, AR Druzhinin, VP Golubev, VB Kravchenko, EA Onuchin, AP Serednyakov, SI Skoypen, YI Solodov, EP Todyshev, KY Yushkov, AN Kirkby, D Lankford, A Mandelkern, M Dey, B Gary, JW Long, O Vitug, GM Campagnari, C Sevilla, MF Hong, TM Kovalskyi, D Richman, JD West, CA Eisner, AM Lockman, WS Martinez, AJ Schumm, BA Seiden, A Chao, DS Cheng, CH Echenard, B Flood, KT Hitlin, DG Ongmongkolkul, P Porter, FC Rakitin, AY Andreassen, R Huard, Z Meadows, BT Sokoloff, MD Sue, L Bloom, PC Ford, WT Gaz, A Nauenberg, U Smith, JG Wagner, SR Ayad, R Toki, WH Spaan, B Schubert, KR Schwierz, R Bernard, D Verderi, M Clark, PJ Playfer, S Bettoni, D Bozzi, C Calabrese, R Cibinetto, G Fioravanti, E Garzia, I Luppi, E Piemontese, L Santoro, V Baldini-Ferroliw, R Calcaterra, A de Sangro, R Finocchiaro, G Patteri, R Peruzzi, IM Piccolo, M Rama, M Zallo, A Contri, R Ab'x, EG Lo Vetere, M Monge, MR Passaggio, S Patrignani, C Robutti, E Bhuyan, B Prasad, V Morii, M Adametz, A Uwer, U Lacker, HM Lueck, T Dauncey, PD Mallik, U Chen, C Cochran, J Meyer, WT Prell, S Rubin, AE Gritsan, AV Arnaud, N Davier, M Derkach, D Grosdidier, G Le Diberder, F Lutz, AM Malaescu, B Roudeau, P Schune, MH Stocchi, A Wormser, G Lange, DJ Wright, DM Burke, JP Coleman, JP Fry, JR Gabathuler, E Gamet, R Hutchcroft, DE Payne, DJ Touramanis, C Bevan, AJ Di Lodovico, E Sacco, R Sigamani, M Cowan, G Brown, DN Davis, CL Denig, AG Fritsch, M Gradl, W Griessinger, K Hafner, A Prencipe, E Barlow, RJ Lafferty, GD Behn, E Cenci, R Hamilton, B Jawahery, A Roberts, DA Dallapiccola, C Cowan, R Dujmic, D Sciolla, G Cheaib, R Patel, PM Robertson, SH Biassoni, R Neri, N Palombo, E Cremaldi, L Godang, R Kroeger, R Sonnek, R Summers, DJ Nguyen, X Simard, M Taras, R De Nardo, G Monorchio, D Onorato, G Sciacca, C Martinelli, M Raven, G Jessop, CP LoSecco, JM Honscheid, K Kass, R Brau, J Frey, R Sinev, NB Strom, D Torrence, E Feltresi, E Gagliardi, N Margoni, M Morandin, M Posocco, M Rotondo, M Simi, G Simonetto, E Stroili, R Akar, S Ben-Haim, E Bomben, M Bonneaud, GR Briand, H Calderini, G Chauveau, J Hamon, O Leruste, P Marchiori, G Ocariz, J Sitt, S Biasini, M Manoni, E Pacetti, S Rossi, A Angelini, C Batignani, G Bettarini, S Carpinelli, M Casarosa, G Cervelli, A Forti, F Giorgi, MA Lusiani, A Oberhof, B Paoloni, E Perez, A Rizzo, G Walsh, J Pegna, DL Olsen, J Smith, AJS Anulli, E Faccini, R Ferrarotto, F Ferroni, E Gaspero, M Gioi, LL Mazzoni, MA Piredda, G Bunger, C Grunberg, O Hartmann, T Leddig, T Voss, C Waldi, R Adye, T Olaiya, EO Wilson, FF Emery, S de Monchenault, GH Vasseur, G Yeche, C Aston, D Bard, DJ Benitez, JF Cartaro, C Convery, MR Dorfan, J Dubois-Felsmann, GP Dunwoodie, W Ebert, M Field, RC Fulsom, BG Gabareen, AM Graham, MT Hast, C Innes, WR Kelsey, MH Kim, P Kocian, ML Leith, DWGS Lewis, R Lindemann, D Lindquist, B Luitz, S Luth, V Lynch, HL MacFarlane, DB Muller, DR Neal, H Nelson, S Perl, M Pulliam, T Ratcliff, BN Roodman, A Salnikov, AA Schindler, RH Snyder, A Su, D Sullivan, MK Va'vra, J Wagner, AP Wang, WF Wisniewski, WJ Wittgen, M Wright, DH Wulsin, HW Ziegler, V Park, W Purohit, MV White, RM Wilson, JR Randle-Conde, A Sekula, SJ Bellis, M Burchat, PR Miyashita, TS Puccio, EMT Alam, MS Ernst, JA Gorodeisky, R Guttman, N Peimer, DR Soffer, A Spanier, SM Ritchie, JL Ruland, AM Schwitters, RF Wray, BC Izen, JM Lou, XC Bianchi, F Gamba, D Zambito, S Lanceri, L Vitale, L Martinez-Vidal, F Oyanguren, A Villanueva-Perez, R Ahmed, H Albert, JJ Banerjee, S Bernlochner, FU Choi, HHF King, GJ Kowalewski, R Lewczuk, MJJ Nugent, IM Roney, JM Sobie, RJ Tasneem, N Gershon, TJ Harrison, PF Latham, TE Band, HR Dasu, S Pan, Y Prepost, R Wu, SL AF Lees, J. P. Poireau, V. Tisserand, V. Grauges, E. Palano, A. Eigen, G. Stugu, B. Brown, D. N. Kerth, Lt. Kolomensky, Yu. G. Lynch, G. Koch, H. Schroeder, T. Asgeirsson, D. J. Hearty, C. Mattison, T. S. McKenna, J. A. So, R. Y. Khan, A. Blinov, V. E. Buzykaev, A. R. Druzhinin, V. P. Golubev, V. B. Kravchenko, E. A. Onuchin, A. P. Serednyakov, S. I. Skoypen, Yu. I. Solodov, E. P. Todyshev, K. Yu. Yushkov, A. N. Kirkby, D. Lankford, At Mandelkern, M. Dey, B. Gary, J. W. Long, O. Vitug, G. M. Campagnari, C. Franco Sevilla, M. Hong, T. M. Kovalskyi, D. Richman, J. D. West, C. A. Eisner, A. M. Lockman, W. S. Martinez, A. J. Schumm, B. A. Seiden, A. Chao, D. S. Cheng, C. H. Echenard, B. Flood, K. T. Hitlin, D. G. Ongmongkolkul, P. Porter, F. C. Rakitin, A. Y. Andreassen, R. Huard, Z. Meadows, B. T. Sokoloff, M. D. Sue, L. Bloom, P. C. Ford, W. T. Gaz, A. Nauenberg, U. Smith, J. G. Wagner, S. R. Ayad, R. Toki, W. H. Spaan, B. Schubert, K. R. Schwierz, R. Bernard, D. Verderi, M. Clark, P. J. Playfer, S. Bettoni, D. Bozzi, C. Calabrese, R. Cibinetto, G. Fioravanti, E. Garzia, I. Luppi, E. Piemontese, L. Santoro, V. Baldini-Ferroliw, R. Calcaterra, A. de Sangro, R. Finocchiaro, G. Patteri, R. Peruzzi, I. M. Piccolo, M. Rama, M. Zallo, A. Contri, R. Guido, E. Lo Vetere, M. Monge, M. R. Passaggio, S. Patrignani, C. Robutti, E. Bhuyan, B. Prasad, V. Morii, M. Adametz, A. Uwer, U. Lacker, H. M. Lueck, T. Dauncey, P. D. Mallik, U. Chen, C. Cochran, J. Meyer, W. T. Prell, S. Rubin, A. E. Gritsan, A. V. Arnaud, N. Davier, M. Derkach, D. Grosdidier, G. Le Diberder, F. Lutz, A. M. Malaescu, B. Roudeau, P. Schune, M. H. Stocchi, A. Wormser, G. Lange, D. J. Wright, D. M. Burke, J. P. Coleman, J. P. Fry, J. R. Gabathuler, E. Gamet, R. Hutchcroft, D. E. Payne, D. J. Touramanis, C. Bevan, A. J. Di Lodovico, E. Sacco, R. Sigamani, M. Cowan, G. Brown, D. N. Davis, C. L. Denig, A. G. Fritsch, M. Gradl, W. Griessinger, K. Hafner, A. Prencipe, E. Barlow, R. J. Lafferty, G. D. Behn, E. Cenci, R. Hamilton, B. Jawahery, A. Roberts, D. A. Dallapiccola, C. Cowan, R. Dujmic, D. Sciolla, G. Cheaib, R. Patel, P. M. Robertson, S. H. Biassoni, R. Neri, N. Palombo, E. Cremaldi, L. Godang, R. Kroeger, R. Sonnek, R. Summers, D. J. Nguyen, X. Simard, M. Taras, R. De Nardo, G. Monorchio, D. Onorato, G. Sciacca, C. Martinelli, M. Raven, G. Jessop, C. P. LoSecco, J. M. Honscheid, K. Kass, R. Brau, J. Frey, R. Sinev, N. B. Strom, D. Torrence, E. Feltresi, E. Gagliardi, N. Margoni, M. Morandin, M. Posocco, M. Rotondo, M. Simi, G. Simonetto, E. Stroili, R. Akar, S. Ben-Haim, E. Bomben, M. Bonneaud, G. R. Briand, H. Calderini, G. Chauveau, J. Hamon, O. Leruste, Ph. Marchiori, G. Ocariz, J. Sitt, S. Biasini, M. Manoni, E. Pacetti, S. Rossi, A. Angelini, C. Batignani, G. Bettarini, S. Carpinelli, M. Casarosa, G. Cervelli, A. Forti, F. Giorgi, M. A. Lusiani, A. Oberhof, B. Paoloni, E. Perez, A. Rizzo, G. Walsh, J. Pegna, D. Lopes Olsen, J. Smith, A. J. S. Anulli, E. Faccini, R. Ferrarotto, F. Ferroni, E. Gaspero, M. Gioi, L. Li Mazzoni, M. A. Piredda, G. Buenger, C. Gruenberg, O. Hartmann, T. Leddig, T. Voss, C. Waldi, R. Adye, T. Olaiya, E. O. Wilson, F. F. Emery, S. de Monchenault, G. Hamel Vasseur, G. Yeche, Ch. Aston, D. Bard, D. J. Benitez, J. F. Cartaro, C. Convery, M. R. Dorfan, J. Dubois-Felsmann, G. P. Dunwoodie, W. Ebert, M. Field, R. C. Fulsom, B. G. Gabareen, A. M. Graham, M. T. Hast, C. Innes, W. R. Kelsey, M. H. Kim, P. Kocian, M. L. Leith, D. W. G. S. Lewis, R. Lindemann, D. Lindquist, B. Luitz, S. Luth, V. Lynch, H. L. MacFarlane, D. B. Muller, D. R. Neal, H. Nelson, S. Perl, M. Pulliam, T. Ratcliff, B. N. Roodman, A. Salnikov, A. A. Schindler, R. H. Snyder, A. Su, D. Sullivan, M. K. Va'vra, J. Wagner, A. P. Wang, W. F. Wisniewski, W. J. Wittgen, M. Wright, D. H. Wulsin, H. W. Ziegler, V. Park, W. Purohit, M. V. White, R. M. Wilson, J. R. Randle-Conde, A. Sekula, S. J. Bellis, M. Burchat, P. R. Miyashita, T. S. Puccio, E. M. T. Alam, M. S. Ernst, J. A. Gorodeisky, R. Guttman, N. Peimer, D. R. Soffer, A. Spanier, S. M. Ritchie, J. L. Ruland, A. M. Schwitters, R. F. Wray, B. C. Izen, J. M. Lou, X. C. Bianchi, F. Gamba, D. Zambito, S. Lanceri, L. Vitale, L. Martinez-Vidal, F. Oyanguren, A. Villanueva-Perez, R. Ahmed, H. Albert, J. J. Banerjee, Sw. Bernlochner, F. U. Choi, H. H. F. King, G. J. Kowalewski, R. Lewczuk, M. J. J. Nugent, I. M. Roney, J. M. Sobie, R. J. Tasneem, N. Gershon, T. J. Harrison, P. F. Latham, T. E. Band, H. R. Dasu, S. Pan, Y. Prepost, R. Wu, S. L. CA BABAR Collaboration TI Time-integrated luminosity recorded by the BABAR detector at the PEP-II e(+)e(-) collider SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE BABAR; Integrated luminosity; Electron-positron collider; PEP-II ID PARTON SHOWER; MONTE-CARLO; ANNIHILATION AB We describe a measurement of the time-integrated luminosity of the data collected by the BABAR experiment at the PEP-II asymmetric-energy e(+)e(-) collider at the Upsilon(4S), Upsilon(3S), and Upsilon(2S) resonances and in a continuum region below each resonance. We measure the time-integrated luminosity by counting e(+)e(-)-> e(+)e(-) and (for the Upsilon(4S) only) e(+)e(-)->mu(+)mu(-) candidate events, allowing additional photons in the final state. We use data-corrected simulation to determine the cross-sections and reconstruction efficiencies for these processes, as well as the major backgrounds. Due to the large cross-sections of e(+)e(-)-> e(+)e(-) and e(+)e(-)->mu(+)mu(-), the statistical uncertainties of the measurement are substantially smaller than the systematic uncertainties. The dominant systematic uncertainties are due to observed differences between data and simulation, as well as uncertainties on the cross-sections. For data collected on the Upsilon(3S) and Upsilon(2S) resonances, an additional uncertainty arises due to Upsilon -> e(+)e(-)X background. For data collected off the Upsilon resonances, we estimate an additional uncertainty due to time dependent efficiency variations, which can affect the short off-resonance runs. The relative uncertainties on the luminosities of the on-resonance (off-resonance) samples are 0.43% (0.43%) for the Upsilon(4S), 0.58% (0.72%) for the Upsilon(3S), and 0.68% (0.88%) for the Upsilon(2S). (C) 2013 Elsevier B.V. All rights reserved. C1 [Lees, J. P.; Poireau, V.; Tisserand, V.; Bettoni, D.; Bozzi, C.; Piemontese, L.; Santoro, V.; Passaggio, S.; Robutti, E.; Neri, N.; Morandin, M.; Posocco, M.; Rotondo, M.; Simi, G.; Perez, A.; Walsh, J.; Anulli, E.; Ferrarotto, F.; Gioi, L. Li; Mazzoni, M. A.; Piredda, G.] Univ Savoie, CNRS IN2P3, LAPP, F-74941 A Le Vieux, France. [Grauges, E.] Univ Barcelona, Fac Fis, Dept ECM, E-08028 Barcelona, Spain. [Palano, A.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Palano, A.] Univ Bari, Dipartimento Fis, I-70126 Bari, Italy. [Eigen, G.; Stugu, B.] Univ Bergen, Inst Phys, N-5007 Bergen, Norway. [Brown, D. N.; Kerth, Lt.; Kolomensky, Yu. G.; Lynch, G.] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Brown, D. N.; Kerth, Lt.; Kolomensky, Yu. G.; Lynch, G.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Koch, H.; Schroeder, T.] Ruhr Univ Bochum, Inst Expt Phys 1, D-44780 Bochum, Germany. [Asgeirsson, D. J.; Hearty, C.; Mattison, T. S.; McKenna, J. A.; So, R. Y.] Univ British Columbia, Vancouver, BC V6T 1Z1, Canada. [Khan, A.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Blinov, V. E.; Buzykaev, A. R.; Druzhinin, V. P.; Golubev, V. B.; Kravchenko, E. A.; Onuchin, A. P.; Serednyakov, S. I.; Skoypen, Yu. I.; Solodov, E. P.; Todyshev, K. Yu.; Yushkov, A. N.] Budker Inst Nucl Phys SB RAS, Novosibirsk 630090, Russia. [Kirkby, D.; Lankford, At; Mandelkern, M.] Univ Calif Irvine, Irvine, CA 92697 USA. [Dey, B.; Gary, J. W.; Long, O.; Vitug, G. M.] Univ Calif Riverside, Riverside, CA 92521 USA. [Campagnari, C.; Franco Sevilla, M.; Hong, T. M.; Kovalskyi, D.; Richman, J. D.; West, C. A.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Eisner, A. M.; Lockman, W. S.; Martinez, A. J.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Inst Particle Phys, Santa Cruz, CA 95064 USA. [Chao, D. S.; Cheng, C. H.; Echenard, B.; Flood, K. T.; Hitlin, D. G.; Ongmongkolkul, P.; Porter, F. C.; Rakitin, A. Y.; Andreassen, R.] CALTECH, Pasadena, CA 91125 USA. [Huard, Z.; Meadows, B. T.; Sokoloff, M. D.; Sue, L.] Univ Cincinnati, Cincinnati, OH 45221 USA. [Bloom, P. C.; Ford, W. T.; Gaz, A.; Nauenberg, U.; Smith, J. G.; Wagner, S. R.; Ayad, R.] Univ Colorado, Boulder, CO 80309 USA. [Toki, W. H.] Colorado State Univ, Ft Collins, CO 80523 USA. [Spaan, B.] Tech Univ Dortmund, Fak Phys, D-44221 Dortmund, Germany. [Schubert, K. R.; Schwierz, R.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Bernard, D.; Verderi, M.] Ecole Polytech, CNRS, IN2P3, Lab Leprince Ringuet, F-91128 Palaiseau, France. [Clark, P. J.; Playfer, S.] Univ Edinburgh, Edinburgh EH9 3JZ, Midlothian, Scotland. [Bettoni, D.; Bozzi, C.; Calabrese, R.; Cibinetto, G.; Fioravanti, E.; Garzia, I.; Luppi, E.; Piemontese, L.; Santoro, V.] Ist Nazl Fis Nucl, Sez Ferrara, I-44100 Ferrara, Italy. [Bettoni, D.; Bozzi, C.; Calabrese, R.; Cibinetto, G.; Fioravanti, E.; Garzia, I.; Luppi, E.; Piemontese, L.; Santoro, V.] Univ Ferrara, Dipartimento Fis, I-44100 Ferrara, Italy. [Baldini-Ferroliw, R.; Calcaterra, A.; de Sangro, R.; Finocchiaro, G.; Patteri, R.; Peruzzi, I. M.; Piccolo, M.; Rama, M.; Zallo, A.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Contri, R.; Guido, E.; Lo Vetere, M.; Monge, M. R.; Passaggio, S.; Patrignani, C.; Robutti, E.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Contri, R.; Guido, E.; Lo Vetere, M.; Monge, M. R.; Passaggio, S.; Patrignani, C.; Robutti, E.] Univ Genoa, Dipartimento Fis, I-16146 Genoa, Italy. [Bhuyan, B.; Prasad, V.] Indian Inst Technol Guwahati, Gauhati 781039, Assam, India. [Morii, M.] Harvard Univ, Cambridge, MA 02138 USA. [Adametz, A.; Uwer, U.] Heidelberg Univ, Inst Phys, D-69120 Heidelberg, Germany. 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R.; Briand, H.; Calderini, G.; Chauveau, J.; Hamon, O.; Leruste, Ph.; Marchiori, G.; Ocariz, J.; Sitt, S.] Univ Paris 07, Univ Paris 06, IN2P3 CNRS, Phys Theor & Hautes Energies Lab, F-75252 Paris, France. [Biasini, M.; Manoni, E.; Pacetti, S.; Rossi, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Biasini, M.; Manoni, E.; Pacetti, S.; Rossi, A.] Univ Perugia, Dipartimento Fis, I-06100 Perugia, Italy. [Angelini, C.; Batignani, G.; Bettarini, S.; Carpinelli, M.; Casarosa, G.; Cervelli, A.; Forti, F.; Giorgi, M. A.; Lusiani, A.; Oberhof, B.; Paoloni, E.; Perez, A.; Rizzo, G.; Walsh, J.] Ist Nazl Fis Nucl, Sez Pisa, I-56127 Pisa, Italy. [Angelini, C.; Batignani, G.; Bettarini, S.; Carpinelli, M.; Casarosa, G.; Cervelli, A.; Forti, F.; Giorgi, M. A.; Lusiani, A.; Oberhof, B.; Paoloni, E.; Perez, A.; Rizzo, G.; Walsh, J.] Univ Pisa, Dipartimento Fis, I-56127 Pisa, Italy. [Angelini, C.; Batignani, G.; Bettarini, S.; Carpinelli, M.; Casarosa, G.; Cervelli, A.; Forti, F.; Giorgi, M. A.; Lusiani, A.; Oberhof, B.; Paoloni, E.; Perez, A.; Rizzo, G.; Walsh, J.] Scuola Normale Super Pisa, I-56127 Pisa, Italy. [Pegna, D. Lopes; Olsen, J.; Smith, A. J. S.] Princeton Univ, Princeton, NJ 08544 USA. [Anulli, E.; Faccini, R.; Ferrarotto, F.; Ferroni, E.; Gaspero, M.; Gioi, L. Li; Mazzoni, M. A.; Piredda, G.] Ist Nazl Fis Nucl, Sez Roma, I-00185 Rome, Italy. [Anulli, E.; Faccini, R.; Ferrarotto, F.; Ferroni, E.; Gaspero, M.; Gioi, L. Li; Mazzoni, M. A.; Piredda, G.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Buenger, C.; Gruenberg, O.; Hartmann, T.; Leddig, T.; Voss, C.; Waldi, R.] Univ Rostock, D-18051 Rostock, Germany. [Adye, T.; Olaiya, E. O.; Wilson, F. F.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Emery, S.; de Monchenault, G. Hamel; Vasseur, G.; Yeche, Ch.] CEA, Irfu, SPP, Ctr Saclay, F-91191 Gif Sur Yvette, France. [Aston, D.; Bard, D. J.; Benitez, J. F.; Cartaro, C.; Convery, M. R.; Dorfan, J.; Dubois-Felsmann, G. P.; Dunwoodie, W.; Ebert, M.; Field, R. C.; Fulsom, B. G.; Gabareen, A. M.; Graham, M. T.; Hast, C.; Innes, W. R.; Kelsey, M. H.; Kim, P.; Kocian, M. L.; Leith, D. W. G. S.; Lewis, R.; Lindquist, B.; Luitz, S.; Luth, V.; Lynch, H. L.; MacFarlane, D. B.; Muller, D. R.; Neal, H.; Nelson, S.; Perl, M.; Pulliam, T.; Ratcliff, B. N.; Roodman, A.; Salnikov, A. A.; Schindler, R. H.; Snyder, A.; Su, D.; Sullivan, M. K.; Va'vra, J.; Wagner, A. P.; Wang, W. F.; Wisniewski, W. J.; Wittgen, M.; Wright, D. H.; Wulsin, H. W.; Ziegler, V.] SLAC Natl Accelerator Lab, Stanford, CA 94309 USA. [Park, W.; Purohit, M. V.; White, R. M.; Wilson, J. R.] Univ S Carolina, Columbia, SC 29208 USA. [Randle-Conde, A.; Sekula, S. J.] So Methodist Univ, Dallas, TX 75275 USA. [Bellis, M.; Burchat, P. R.; Miyashita, T. S.; Puccio, E. M. T.; Alam, M. S.] Stanford Univ, Stanford, CA 94305 USA. [Ernst, J. A.] SUNY Albany, Albany, NY 12222 USA. [Gorodeisky, R.; Guttman, N.; Peimer, D. R.; Soffer, A.] Tel Aviv Univ, Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Spanier, S. M.] Univ Tennessee, Knoxville, TN 37996 USA. [Ritchie, J. L.; Ruland, A. M.; Schwitters, R. F.; Wray, B. C.] Univ Texas Austin, Austin, TX 78712 USA. [Izen, J. M.; Lou, X. C.] Univ Texas Dallas, Richardson, TX 75083 USA. [Bianchi, F.; Gamba, D.; Zambito, S.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Bianchi, F.; Gamba, D.; Zambito, S.] Univ Turin, Dipartimento Fis Sperimentale, I-10125 Turin, Italy. [Lindemann, D.; Lanceri, L.; Vitale, L.] Ist Nazl Fis Nucl, Sez Trieste, I-34127 Trieste, Italy. [Lindemann, D.; Lanceri, L.; Vitale, L.] Univ Trieste, Dipartimento Fis, I-34127 Trieste, Italy. [Martinez-Vidal, F.; Oyanguren, A.; Villanueva-Perez, R.] Univ Valencia, CSIC, IFIC, E-46071 Valencia, Spain. [Ahmed, H.; Albert, J. J.; Banerjee, Sw.; Bernlochner, F. U.; Choi, H. H. F.; King, G. J.; Kowalewski, R.; Lewczuk, M. J. J.; Nugent, I. M.; Roney, J. M.; Sobie, R. J.; Tasneem, N.] Univ Victoria, Victoria, BC V8W 3P6, Canada. [Gershon, T. J.; Harrison, P. F.; Latham, T. E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Band, H. R.; Dasu, S.; Pan, Y.; Prepost, R.; Wu, S. L.] Univ Wisconsin, Madison, WI 53706 USA. [Peruzzi, I. M.] Univ Perugia, Dipartimento Fis, I-06100 Perugia, Italy. [Carpinelli, M.] Univ Sassari, I-07100 Sassari, Italy. RP Soffer, A (reprint author), Tel Aviv Univ, Sch Phys & Astron, IL-69978 Tel Aviv, Israel. EM abi@slac.stanford.edu RI Forti, Francesco/H-3035-2011; Oyanguren, Arantza/K-6454-2014; Luppi, Eleonora/A-4902-2015; White, Ryan/E-2979-2015; Kravchenko, Evgeniy/F-5457-2015; Calabrese, Roberto/G-4405-2015; Martinez Vidal, F*/L-7563-2014; Kolomensky, Yury/I-3510-2015; Lo Vetere, Maurizio/J-5049-2012; Lusiani, Alberto/N-2976-2015; Patrignani, Claudia/C-5223-2009; Monge, Maria Roberta/G-9127-2012; Morandin, Mauro/A-3308-2016; Lusiani, Alberto/A-3329-2016; Di Lodovico, Francesca/L-9109-2016; Calcaterra, Alessandro/P-5260-2015; Frey, Raymond/E-2830-2016; Rizzo, Giuliana/A-8516-2015; OI Forti, Francesco/0000-0001-6535-7965; Oyanguren, Arantza/0000-0002-8240-7300; Luppi, Eleonora/0000-0002-1072-5633; White, Ryan/0000-0003-3589-5900; Calabrese, Roberto/0000-0002-1354-5400; Martinez Vidal, F*/0000-0001-6841-6035; Kolomensky, Yury/0000-0001-8496-9975; Lo Vetere, Maurizio/0000-0002-6520-4480; Lusiani, Alberto/0000-0002-6876-3288; Patrignani, Claudia/0000-0002-5882-1747; Monge, Maria Roberta/0000-0003-1633-3195; Morandin, Mauro/0000-0003-4708-4240; Lusiani, Alberto/0000-0002-6876-3288; Di Lodovico, Francesca/0000-0003-3952-2175; Calcaterra, Alessandro/0000-0003-2670-4826; Frey, Raymond/0000-0003-0341-2636; Lanceri, Livio/0000-0001-8220-3095; Ebert, Marcus/0000-0002-3014-1512; Paoloni, Eugenio/0000-0001-5969-8712; Cibinetto, Gianluigi/0000-0002-3491-6231; Pacetti, Simone/0000-0002-6385-3508; Sciacca, Crisostomo/0000-0002-8412-4072; Rizzo, Giuliana/0000-0003-1788-2866; Martinelli, Maurizio/0000-0003-4792-9178; Faccini, Riccardo/0000-0003-2613-5141; Chen, Chunhui /0000-0003-1589-9955; Bellis, Matthew/0000-0002-6353-6043 FU US Department of Energy and National Science Foundation; Natural Sciences and Engineering Research Council (Canada); Commissariat a l'Energie Atomique and Institut National de Physique Nucleaire et de Physique des Particules (France); Bundesministerium fur Bildung und Forschung and Deutsche Forschungsgemeinschaft (Germany); Istituto Nazionale di Fisica Nucleare (Italy); Foundation for Fundamental Research on Matter (The Netherlands); Research Council of Norway; Ministry of Education and Science of the Russian Federation; Ministerio de Ciencia e Innovacion (Spain); Science and Technology Facilities Council (United Kingdom); Marie-Curie IEF program (European Union); A. P. Sloan Foundation (USA) FX We are grateful for the extraordinary contributions of our PEP-II colleagues in achieving the excellent luminosity and machine conditions that have made this work possible. The success of this project also relies critically on the expertise and dedication of the computing organizations that support BABAR. The collaborating institutions wish to thank SLAC for its support and the kind hospitality extended to them. This work is supported by the US Department of Energy and National Science Foundation, the Natural Sciences and Engineering Research Council (Canada), the Commissariat a l'Energie Atomique and Institut National de Physique Nucleaire et de Physique des Particules (France), the Bundesministerium fur Bildung und Forschung and Deutsche Forschungsgemeinschaft (Germany), the Istituto Nazionale di Fisica Nucleare (Italy), the Foundation for Fundamental Research on Matter (The Netherlands), the Research Council of Norway, the Ministry of Education and Science of the Russian Federation, Ministerio de Ciencia e Innovacion (Spain), and the Science and Technology Facilities Council (United Kingdom). Individuals have received support from the Marie-Curie IEF program (European Union) and the A. P. Sloan Foundation (USA). NR 15 TC 48 Z9 48 U1 2 U2 29 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD OCT 21 PY 2013 VL 726 BP 203 EP 213 DI 10.1016/j.nima.2013.04.029 PG 11 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 206WU UT WOS:000323557200028 ER PT J AU Vilcaez, J Li, L Wu, DH Hubbard, SS AF Vilcaez, Javier Li, Li Wu, Dinghao Hubbard, Susan S. TI Reactive Transport Modeling of Induced Selective Plugging by Leuconostoc Mesenteroides in Carbonate Formations SO GEOMICROBIOLOGY JOURNAL LA English DT Article DE enhanced oil recovery; modeling; permeability modification; reactive transport; selective plugging ID SATURATED HYDRAULIC CONDUCTIVITY; ENHANCED OIL-RECOVERY; POROUS-MEDIA; HYDROTHERMAL SYSTEMS; PROFILE MODIFICATION; CHEMICAL-REACTIONS; AQUIFER MATERIALS; ROCK INTERACTIONS; MICROBIAL-GROWTH; MASS-TRANSPORT AB A process-based mechanistic reactive transport model was developed to understand how in-situ coupled processes and operational factors affect selective plugging of reactive carbonate formations by the fermenting bacteria Leuconostoc mesenteroides that produces a plugging polymer dextran. The growth and transport of L. mesenteroides and the associated (bio) geochemical reactions were simulated explicitly with enzyme activity at the field scale over spatial extents of hundreds of meters. Simulations were performed to explore controls on selective bioplugging of high permeability zones in a representative carbonate reservoir, a process that can be used to improve oil sweep efficiency through lower permeability layers. Simulation results indicate that dextran production and the effectiveness of plugging can be largely affected by sucrose and bacteria injection rates. Selective plugging of high permeability zones can only be achieved when the injection rates are high compared to the rates of dextran production. Otherwise, plugging only occurs at the vicinity of injection wells. Due to the dependence of enzyme activity on pH and the reactive nature of carbonate formations, the chemistry of the injection and the formation water is also important. The injection of sucrose and L. mesenteroides at the optimum pH for dextran production (5.2) leads to the dissolution of calcite and an increase in pH levels. However, the resulting pH does not suppress plugging with dextran. Lactic acid and CO2 formed during the growth of L. mesenteroides buffers the pH of water to levels between 5.2 and 7.0 for continued dextran production. At neutral and basic pH levels, induced precipitation of calcite does not significantly modify the permeability profile at carbonate concentrations typically found in oilfield formation waters. This is the first work that examines the controlling parameters that affect selective plugging of carbonate formations at the field scale within the context of enhanced oil recovery. The demonstrated approach can be used to identify optimal operational conditions for enhanced oil recovery and other applications where selective plugging can be beneficial. C1 [Vilcaez, Javier; Li, Li] Penn State Univ, John & Willie Leone Family Dept Energy & Mineral, University Pk, PA 16802 USA. [Vilcaez, Javier; Li, Li] Penn State Univ, EMS Energy Inst, University Pk, PA 16802 USA. [Li, Li] Penn State Univ, Earth & Environm Syst Inst EESI, University Pk, PA 16802 USA. [Wu, Dinghao] Penn State Univ, Coll Informat Sci & Technol, University Pk, PA 16802 USA. [Hubbard, Susan S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Vilcaez, J (reprint author), Univ Tokyo, Fac Engn, Bunkyo Ku, 7-3-1 Hongo, Tokyo 1138656, Japan. EM vilcaez@frcer.t.u-tokyo.ac.jp RI Hubbard, Susan/E-9508-2010; Li, Li/A-6077-2008 OI Li, Li/0000-0002-1641-3710 FU University of California at Berkeley, Energy Biosciences Institute; BP FX This work was supported by the University of California at Berkeley, Energy Biosciences Institute to Pennsylvania State University. The Energy Biosciences Institute is funded by BP. NR 82 TC 9 Z9 9 U1 1 U2 40 PU TAYLOR & FRANCIS INC PI PHILADELPHIA PA 325 CHESTNUT ST, SUITE 800, PHILADELPHIA, PA 19106 USA SN 0149-0451 J9 GEOMICROBIOL J JI Geomicrobiol. J. PD OCT 21 PY 2013 VL 30 IS 9 BP 813 EP 828 DI 10.1080/01490451.2013.774074 PG 16 WC Environmental Sciences; Geosciences, Multidisciplinary SC Environmental Sciences & Ecology; Geology GA 189ZW UT WOS:000322307800004 ER PT J AU Vilcaez, J Li, L Hubbard, SS AF Vilcaez, Javier Li, Li Hubbard, Susan S. TI A new model for the biodegradation kinetics of oil droplets: application to the Deepwater Horizon oil spill in the Gulf of Mexico SO GEOCHEMICAL TRANSACTIONS LA English DT Article DE Modeling; Biodegradation; Oil droplets; Size distribution; Shrinking core model; Gulf of Mexico oil spill; Deepwater horizon oil spill ID CHEMICAL DISPERSANT EFFECTIVENESS; PARTICLE-SIZE DISTRIBUTION; TRUE YIELD PREDICTION; PSEUDOMONAS-PUTIDA F1; CRUDE-OIL; P-XYLENE; BENZENE; TOLUENE; MIXTURES; BACTERIA AB Oil biodegradation by native bacteria is one of the most important natural processes that can attenuate the environmental impacts of marine oil spills. Existing models for oil biodegradation kinetics are mostly for dissolved oil. This work developed a new mathematical model for the biodegradation of oil droplets and applied the model to estimate the time scale for oil biodegradation under conditions relevant to the Deepwater Horizon oil spill in the Gulf of Mexico. In the model, oil is composed of droplets of various sizes following the gamma function distribution. Each oil droplet shrinks during the microbe-mediated degradation at the oil-water interface. Using our developed model, we find that the degradation of oil droplets typically goes through two stages. The first stage is characterized by microbial activity unlimited by oil-water interface with higher biodegradation rates than that of the dissolved oil. The second stage is governed by the availability of the oil-water interface, which results in much slower rates than that of soluble oil. As a result, compared to that of the dissolved oil, the degradation of oil droplets typically starts faster and then quickly slows down, ultimately reaching a smaller percentage of degraded oil in longer time. The availability of the water-oil interface plays a key role in determining the rates and extent of degradation. We find that several parameters control biodegradation rates, including size distribution of oil droplets, initial microbial concentrations, initial oil concentration and composition. Under conditions relevant to the Deepwater Horizon spill, we find that the size distribution of oil droplets (mean and coefficient of variance) is the most important parameter because it determines the availability of the oil-water interface. Smaller oil droplets with larger variance leads to faster and larger extent of degradation. The developed model will be useful for evaluating transport and fate of spilled oil, different remediation strategies, and risk assessment. C1 [Vilcaez, Javier; Li, Li] Penn State Univ, John & Willie Leone Family Dept Energy & Mineral, University Pk, PA 16802 USA. [Vilcaez, Javier; Li, Li] Penn State Univ, EMS Energy Inst, University Pk, PA 16802 USA. [Li, Li] Penn State Univ, EESI, University Pk, PA 16802 USA. [Hubbard, Susan S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Li, L (reprint author), Penn State Univ, John & Willie Leone Family Dept Energy & Mineral, University Pk, PA 16802 USA. EM lili@eme.psu.edu RI Hubbard, Susan/E-9508-2010; Li, Li/A-6077-2008 OI Li, Li/0000-0002-1641-3710 FU University of California at Berkeley, Energy Biosciences Institute under its U.S. Department of Energy [DE-AC02-05CH11231]; BP FX This work was supported by a subcontract from the University of California at Berkeley, Energy Biosciences Institute, to Lawrence Berkeley National Laboratory under its U.S. Department of Energy contract DE-AC02-05CH11231. The Energy Biosciences Institute is funded by BP. NR 55 TC 7 Z9 7 U1 7 U2 47 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1467-4866 J9 GEOCHEM T JI Geochem. Trans. PD OCT 20 PY 2013 VL 14 AR 4 DI 10.1186/1467-4866-14-4 PG 14 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA 273PB UT WOS:000328546600001 PM 24138161 ER PT J AU Archambault, S Arlen, T Aune, T Behera, B Beilicke, M Benbow, W Bird, R Bouvier, A Buckley, JH Bugaev, V Byrum, K Cesarini, A Ciupik, L Connolly, MP Cui, W Errando, M Falcone, A Federici, S Feng, Q Finley, JP Fortson, L Furniss, A Galante, N Gall, D Gillanders, GH Griffin, S Grube, J Gyuk, G Hanna, D Holder, J Hughes, G Humensky, TB Kaaret, P Kertzman, M Khassen, Y Kieda, D Krawczynski, H Krennrich, F Kumar, S Lang, MJ Madhavan, AS Maier, G Majumdar, P McArthur, S McCann, A Millis, J Moriarty, P Mukherjee, R de Bhroithe, AO Ong, RA Otte, AN Park, N Perkins, JS Pohl, M Popkow, A Prokoph, H Quinn, J Ragan, K Reyes, LC Reynolds, PT Richards, GT Roache, E Saxon, DB Sembroski, GH Smith, AW Staszak, D Telezhinsky, I Theiling, M Varlotta, A Vassiliev, VV Vincent, S Wakely, SP Weekes, TC Weinstein, A Welsing, R Williams, DA Zitzer, B Bottcher, M Fegan, SJ Fortin, P Halpern, JP Kovalev, YY Lister, ML Liu, J Pushkarev, AB Smith, PS AF Archambault, S. Arlen, T. Aune, T. Behera, B. Beilicke, M. Benbow, W. Bird, R. Bouvier, A. Buckley, J. H. Bugaev, V. Byrum, K. Cesarini, A. Ciupik, L. Connolly, M. P. Cui, W. Errando, M. Falcone, A. Federici, S. Feng, Q. Finley, J. P. Fortson, L. Furniss, A. Galante, N. Gall, D. Gillanders, G. H. Griffin, S. Grube, J. Gyuk, G. Hanna, D. Holder, J. Hughes, G. Humensky, T. B. Kaaret, P. Kertzman, M. Khassen, Y. Kieda, D. Krawczynski, H. Krennrich, F. Kumar, S. Lang, M. J. Madhavan, A. S. Maier, G. Majumdar, P. McArthur, S. McCann, A. Millis, J. Moriarty, P. Mukherjee, R. de Bhroithe, A. O'Faolain Ong, R. A. Otte, A. N. Park, N. Perkins, J. S. Pohl, M. Popkow, A. Prokoph, H. Quinn, J. Ragan, K. Reyes, L. C. Reynolds, P. T. Richards, G. T. Roache, E. Saxon, D. B. Sembroski, G. H. Smith, A. W. Staszak, D. Telezhinsky, I. Theiling, M. Varlotta, A. Vassiliev, V. V. Vincent, S. Wakely, S. P. Weekes, T. C. Weinstein, A. Welsing, R. Williams, D. A. Zitzer, B. Boettcher, M. Fegan, S. J. Fortin, P. Halpern, J. P. Kovalev, Y. Y. Lister, M. L. Liu, J. Pushkarev, A. B. Smith, P. S. CA VERITAS Collaboration TI DISCOVERY OF A NEW TeV GAMMA-RAY SOURCE: VER J0521+211 SO ASTROPHYSICAL JOURNAL LA English DT Article DE BL Lacertae objects: individual (VER J0521+211); gamma rays: galaxies ID ACTIVE GALACTIC NUCLEI; LARGE-AREA TELESCOPE; EXTRAGALACTIC BACKGROUND LIGHT; ALL-SKY SURVEY; HIGH-ENERGY EMISSION; MULTIWAVELENGTH OBSERVATIONS; SOURCE CATALOG; BL-LAC; LINEAR-POLARIZATION; DETECTED BLAZARS AB We report the detection of a new TeV gamma-ray source, VER J0521+211, based on observations made with the VERITAS imaging atmospheric Cherenkov Telescope Array. These observations were motivated by the discovery of a cluster of >30 GeV photons in the first year of Fermi Large Area Telescope observations. VER J0521+211 is relatively bright at TeV energies, with a mean photon flux of (1.93 +/- 0.13(stat) +/- 0.78(sys)) x 10(-11) cm(-2) s(-1) above 0.2 TeV during the period of the VERITAS observations. The source is strongly variable on a daily timescale across all wavebands, from optical to TeV, with a peak flux corresponding to similar to 0.3 times the steady Crab Nebula flux at TeV energies. Follow-up observations in the optical and X-ray bands classify the newly discovered TeV source as a BL Lac-type blazar with uncertain redshift, although recent measurements suggest z = 0.108. VER J0521+211 exhibits all the defining properties of blazars in radio, optical, X-ray, and gamma-ray wavelengths. C1 [Archambault, S.; Griffin, S.; Hanna, D.; Ragan, K.; Staszak, D.] McGill Univ, Dept Phys, Montreal, PQ H3A 2T8, Canada. [Arlen, T.; Aune, T.; Majumdar, P.; Ong, R. A.; Popkow, A.; Vassiliev, V. V.] Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA. [Behera, B.; Federici, S.; Hughes, G.; Krawczynski, H.; Maier, G.; Pohl, M.; Prokoph, H.; Telezhinsky, I.; Vincent, S.; Welsing, R.] DESY, D-15738 Zeuthen, Germany. [Beilicke, M.; Buckley, J. H.; Bugaev, V.] Washington Univ, Dept Phys, St Louis, MO 63130 USA. [Benbow, W.; Galante, N.; Roache, E.; Weekes, T. C.; Fortin, P.] Harvard Smithsonian Ctr Astrophys, Fred Lawrence Whipple Observ, Amado, AZ 85645 USA. [Bird, R.; Khassen, Y.; de Bhroithe, A. O'Faolain; Quinn, J.] Univ Coll Dublin, Sch Phys, Dublin 4, Ireland. [Bouvier, A.; Furniss, A.; Williams, D. A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Bouvier, A.; Furniss, A.; Williams, D. A.] Univ Calif Santa Cruz, Dept Phys, Santa Cruz, CA 95064 USA. [Byrum, K.; Zitzer, B.] Argonne Natl Lab, Argonne, IL 60439 USA. [Cesarini, A.; Connolly, M. P.; Gillanders, G. H.; Lang, M. J.] Natl Univ Ireland Galway, Sch Phys, Galway, Ireland. [Ciupik, L.; Grube, J.; Gyuk, G.] Adler Planetarium & Astron Museum, Dept Astron, Chicago, IL 60605 USA. [Cui, W.; Feng, Q.; Finley, J. P.; Sembroski, G. H.; Theiling, M.; Varlotta, A.] Purdue Univ, Dept Phys, W Lafayette, IN 47907 USA. [Errando, M.; Mukherjee, R.] Columbia Univ, Barnard Coll, Dept Phys & Astron, New York, NY 10027 USA. [Falcone, A.] Penn State Univ, Dept Astron & Astrophys, Davey Lab 525, University Pk, PA 16802 USA. [Federici, S.; Pohl, M.; Telezhinsky, I.] Univ Potsdam, Inst Phys & Astron, D-14476 Potsdam, Germany. [Fortson, L.] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Gall, D.; Kaaret, P.] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. [Holder, J.; Kumar, S.; Saxon, D. B.] Univ Delaware, Dept Phys & Astron, Newark, DE 19716 USA. [Holder, J.; Kumar, S.; Saxon, D. B.] Univ Delaware, Bartol Res Inst, Newark, DE 19716 USA. [Humensky, T. B.] Columbia Univ, Dept Phys, New York, NY 10027 USA. [Kertzman, M.] Depauw Univ, Dept Phys & Astron, Greencastle, IN 46135 USA. [Kieda, D.; Smith, A. W.] Univ Utah, Dept Phys & Astron, Salt Lake City, UT 84112 USA. [Krennrich, F.; Madhavan, A. S.; Weinstein, A.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Majumdar, P.] Saha Inst Nucl Phys, Kolkata 700064, India. [McArthur, S.; Park, N.; Wakely, S. P.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [McCann, A.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Millis, J.] Anderson Univ, Dept Phys, Anderson, IN 46012 USA. [Moriarty, P.] Galway Mayo Inst Technol, Dept Life & Phys Sci, Dublin, Ireland. [Otte, A. N.; Richards, G. T.] Georgia Inst Technol, Sch Phys, Atlanta, GA 30332 USA. [Otte, A. N.; Richards, G. T.] Georgia Inst Technol, Ctr Relativist Astrophys, Atlanta, GA 30332 USA. [Perkins, J. S.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Reyes, L. C.] Calif Polytech State Univ San Luis Obispo, Dept Phys, San Luis Obispo, CA 94307 USA. [Reynolds, P. T.] Cork Inst Technol, Dept Appl Phys & Instrumentat, Cork, Ireland. [Boettcher, M.] North West Univ, Ctr Space Res, ZA-2531 Potchefstroom, South Africa. [Fegan, S. J.] Ecole Polytech, CNRS, Lab Leprince Ringuet, F-91128 Palaiseau, France. [Halpern, J. P.; Liu, J.] Columbia Univ, Columbia Astrophys Lab, New York, NY 10027 USA. [Kovalev, Y. Y.] Max Planck Inst Radioastron, D-53121 Bonn, Germany. [Kovalev, Y. Y.] PN Lebedev Phys Inst, Ctr Astro Space, Moscow 117997, Russia. [Lister, M. L.] Purdue Univ, Dept Phys, W Lafayette, IN 47907 USA. [Pushkarev, A. B.] Pulkovo Astron Observ, St Petersburg 196140, Russia. [Pushkarev, A. B.] Crimean Astrophys Observ, UA-98409 Nauchnyi, Crimea, Ukraine. [Smith, P. S.] Univ Arizona, Steward Observ, Tucson, AZ 85721 USA. RP Archambault, S (reprint author), McGill Univ, Dept Phys, 3600 Univ St, Montreal, PQ H3A 2T8, Canada. EM errando@astro.columbia.edu; jholder@physics.udel.edu; sfegan@llr.in2p3.fr; fortin@veritas.sao.arizona.edu RI Kovalev, Yuri/J-5671-2013; Khassen, Yerbol/I-3806-2015; Pushkarev, Alexander/M-9997-2015; OI Kovalev, Yuri/0000-0001-9303-3263; Khassen, Yerbol/0000-0002-7296-3100; Smith, Paul/0000-0002-5083-3663; Cui, Wei/0000-0002-6324-5772; Cesarini, Andrea/0000-0002-8611-8610; Liu, Jia/0000-0001-8219-1995; Errando, Manel/0000-0002-1853-863X; Lang, Mark/0000-0003-4641-4201; Bird, Ralph/0000-0002-4596-8563 FU U.S. Department of Energy Office of Science; U.S. National Science Foundation; Smithsonian Institution; NSERC in Canada; Science Foundation Ireland [SFI 10/RFP/AST2748]; STFC in the UK; INAF in Italy; CNES in France; NASA [NNX10AP66G, NNX12AJ30G, NNX10AF89G]; Russian Foundation for Basic Research [11-02-00368, 12-02-33101]; Russian Academy of Sciences; Dynasty Foundation; South African Department of Science and Technology through the National Research Foundation under NRF SARChI Chair [64789]; NASA-Fermi [NNX08AV67G, 11-Fermi11-0019, NNX09AU10G] FX VERITAS is supported by grants from the U.S. Department of Energy Office of Science, the U.S. National Science Foundation, and the Smithsonian Institution, by NSERC in Canada, by Science Foundation Ireland (SFI 10/RFP/AST2748), and by STFC in the UK. We acknowledge the excellent work of the technical support staff at the Fred Lawrence Whipple Observatory and at the collaborating institutions in the construction and operation of the instrument.; The Fermi-LAT Collaboration acknowledges support from a number of agencies and institutes for both development and the operation of the LAT as well as scientific data analysis. These include NASA and DOE in the United States, CEA/Irfu and IN2P3/CNRS in France, ASI and INFN in Italy, MEXT, KEK, and JAXA in Japan, and the K. A. Wallenberg Foundation, the Swedish Research Council, and the National Space Board in Sweden. Additional support from INAF in Italy and CNES in France for science analysis during the operations phase is also gratefully acknowledged.; M. E. acknowledges support from the NASA grants NNX10AP66G and NNX12AJ30G. Y.Y.K. was supported in part by the Russian Foundation for Basic Research (projects 11-02-00368 and 12-02-33101), the basic research program "Active Processes in Galactic and Extragalactic Objects" of the Physical Sciences Division of the Russian Academy of Sciences, and the Dynasty Foundation. M. B. acknowledges support by the South African Department of Science and Technology through the National Research Foundation under NRF SARChI Chair grant No. 64789.; This research has made use of data from the MOJAVE database that is maintained by the MOJAVE team (Lister et al. 2009a). The MOJAVE project is supported under NASA-Fermi grants NNX08AV67G and 11-Fermi11-0019. The authors thank Julie Skinner for obtaining, as a target of opportunity, the first MDM spectrum of RGB J0521.8+2112 used in this paper, and Talvikki Hovatta for providing the OVRO radio data. Observations at Steward Observatory were supported by the NASA Fermi Guest Investigator Program grant NNX09AU10G. Finally, the authors thank the Swift team for accepting and carefully scheduling the target of opportunity observations of VER J0521+211 that were used in the paper and for support from the Swift Guest Investigator program, NASA grant NNX10AF89G. NR 93 TC 12 Z9 13 U1 0 U2 9 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD OCT 20 PY 2013 VL 776 IS 2 AR 69 DI 10.1088/0004-637X/776/2/69 PG 10 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 255CF UT WOS:000327216100006 ER PT J AU Kucharek, H Fuselier, SA Wurz, P Pogorelov, N Borovikov, S Lee, MA Moebius, E Reisenfeld, D Funsten, H Schwadron, N McComas, D AF Kucharek, H. Fuselier, S. A. Wurz, P. Pogorelov, N. Borovikov, S. Lee, M. A. Moebius, E. Reisenfeld, D. Funsten, H. Schwadron, N. McComas, D. TI THE SOLAR WIND AS A POSSIBLE SOURCE OF FAST TEMPORAL VARIATIONS OF THE HELIOSPHERIC RIBBON SO ASTROPHYSICAL JOURNAL LA English DT Article DE ISM: atoms; ISM: magnetic fields; shock waves; solar wind ID INTERSTELLAR-BOUNDARY-EXPLORER; TERMINATION SHOCK; MAGNETIC-FIELD; OUTER HELIOSPHERE; PICKUP IONS; HELIOSHEATH; VOYAGER-1; FLUX; HELIOPAUSE; DIRECTION AB We present a possible source of pickup ions (PUIs) the ribbon observed by the Interstellar Boundary EXplorer (IBEX). We suggest that a gyrating solar wind and PUIs in the ramp and in the near downstream region of the termination shock (TS) could provide a significant source of energetic neutral atoms (ENAs) in the ribbon. A fraction of the solar wind and PUIs are reflected and energized during the first contact with the TS. Some of the solar wind may be reflected propagating toward the Sun but most of the solar wind ions form a gyrating beam-like distribution that persists until it is fully thermalized further downstream. Depending on the strength of the shock, these gyrating distributions can exist for many gyration periods until they are scattered/thermalized due to wave-particle interactions at the TS and downstream in the heliosheath. During this time, ENAs can be produced by charge exchange of interstellar neutral atoms with the gyrating ions. In order to determine the flux of energetic ions, we estimate the solar wind flux at the TS using pressure estimates inferred from in situ measurements. Assuming an average path length in the radial direction of the order of a few AU before the distribution of gyrating ions is thermalized, one can explain a significant fraction of the intensity of ENAs in the ribbon observed by IBEX. With a localized source and such a short integration path, this model would also allow fast time variations of the ENA flux. C1 [Kucharek, H.; Lee, M. A.; Moebius, E.; Schwadron, N.] Univ New Hampshire, Ctr Space Sci, Durham, NH 03824 USA. [Fuselier, S. A.; McComas, D.] SW Res Inst, San Antonio, TX USA. [Fuselier, S. A.; McComas, D.] Univ Texas San Antonio, Dept Phys, San Antonio, TX USA. [Wurz, P.] Univ Bern, Inst Phys, Bern, Switzerland. [Pogorelov, N.; Borovikov, S.] Univ Alabama, Dept Phys, Huntsville, AL 35899 USA. [Pogorelov, N.; Borovikov, S.] Univ Alabama, Ctr Space Plasma & Aeron Res, Huntsville, AL 35899 USA. [Reisenfeld, D.] Univ Montana, Dept Phys & Astron, Missoula, MT 59812 USA. [Funsten, H.] Los Alamos Natl Lab, Ctr Space Sci & Explorat, Los Alamos, NM USA. RP Kucharek, H (reprint author), Univ New Hampshire, Ctr Space Sci, Durham, NH 03824 USA. EM harald.kucharek@unh.edu RI Funsten, Herbert/A-5702-2015; Reisenfeld, Daniel/F-7614-2015; OI Funsten, Herbert/0000-0002-6817-1039; Moebius, Eberhard/0000-0002-2745-6978 FU NASA [NNX09AG62G]; IBEX mission, which is part of NASA's Explorer Program FX The authors thank E. Roelof for very useful discussions and support for interpreting Voyager data. This work was supported by NASA grant NNX09AG62G and the IBEX mission, which is part of NASA's Explorer Program. NR 37 TC 12 Z9 12 U1 0 U2 4 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD OCT 20 PY 2013 VL 776 IS 2 AR 109 DI 10.1088/0004-637X/776/2/109 PG 13 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 255CF UT WOS:000327216100046 ER PT J AU Jabeen, S AF Jabeen, Shabnam TI TOP AND HIGGS PHYSICS AT THE HADRON COLLIDERS SO INTERNATIONAL JOURNAL OF MODERN PHYSICS A LA English DT Review DE Top quark; Higgs boson; Tevatron; CDF; DO, LHC; CMS; ATLAS ID QUARK-PAIR PRODUCTION; PRODUCTION CROSS-SECTION; PROTON-PROTON COLLISIONS; PLUS JETS CHANNEL; W-GLUON FUSION; ABELIAN GAUGE-THEORIES; DILEPTON FINAL-STATES; ANOMALOUS WTB COUPLINGS; BOOSTED DECISION TREES; NLO QCD CORRECTIONS AB This review summarizes the recent results for top quark and Higgs boson measurements from experiments at Tevatron, a proton-antiproton collider at a center-of-mass energy of root s = 1.96 TeV, and the Large Hadron Collider, a proton-proton collider at a center-of-mass energy of root s = 7 TeV. These results include the discovery of a Higgs-like boson and measurement of its various properties, and measurements in the top quark sector, e. g. top quark mass, spin, charge asymmetry and production of single top quark. C1 Fermilab Natl Accelerator Lab, Batavia, IL USA. RP Jabeen, S (reprint author), Fermilab Natl Accelerator Lab, POB 352, Batavia, IL USA. EM jabeen@fnal.gov NR 487 TC 3 Z9 3 U1 4 U2 32 PU WORLD SCIENTIFIC PUBL CO PTE LTD PI SINGAPORE PA 5 TOH TUCK LINK, SINGAPORE 596224, SINGAPORE SN 0217-751X EI 1793-656X J9 INT J MOD PHYS A JI Int. J. Mod. Phys. A PD OCT 20 PY 2013 VL 28 IS 26 AR UNSP 1330038 DI 10.1142/S0217751X1330038X PG 65 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA 243BI UT WOS:000326291000002 ER PT J AU Drachenberg, DR Andrusyak, O Venus, G Smirnov, V Lumeau, J Glebov, LB AF Drachenberg, Derrek R. Andrusyak, Oleksiy Venus, George Smirnov, Vadim Lumeau, Julien Glebov, Leonid B. TI Ultimate efficiency of spectral beam combining by volume Bragg gratings SO APPLIED OPTICS LA English DT Article ID FIBER AMPLIFIERS; ORDER-MODE; POWER; PROPAGATION; DIFFRACTION; LIGHT; ARRAY; GLASS AB Spectral beam combining (SBC) by volume Bragg gratings (VBGs) recorded in photo-thermo-refractive (PTR) glass is a powerful tool for laser applications that require higher radiance than a single laser unit can achieve. The beam-combining factor (BCF) is introduced as a tool to compare various beam-combining methods and experiments. It describes the change of radiance provided by a beam-combining system but is not affected by the initial beam quality of the combined lasers. A method of optimization of VBGs providing the maximum efficiency of SBC has been described for an arbitrary number of beams. An experiment confirming the proposed modeling for a two-beam SBC system by a single VBG has demonstrated a total combined power of 301 W with a channel separation of 0.25 nm, combining efficiency of 97%, close to diffraction limited divergence with M-2 = 1.18, BCF of 0.77, and spectral radiance of 770 TW/(sr.m(2).nm), the highest to date for SBC. (C) 2013 Optical Society of America C1 [Drachenberg, Derrek R.; Andrusyak, Oleksiy; Venus, George; Lumeau, Julien; Glebov, Leonid B.] Univ Cent Florida, CREOL, Coll Opt & Photon, Orlando, FL 32816 USA. [Smirnov, Vadim] OptiGrate Corp, Oviedo, FL 32765 USA. RP Drachenberg, DR (reprint author), Lawrence Livermore Natl Lab, NIF Photon Sci & Applicat, 7000 East Ave, Livermore, CA 94551 USA. EM drachenberg1@llnl.gov RI Lumeau, Julien/P-6704-2015 OI Lumeau, Julien/0000-0001-9800-4189 FU Defense Advanced Research Projects Agency (DARPA), AD-HELS Program [H0011-06-1-0010]; Directed Energy Professional Society (DEPS) Graduate Scholarship FX This research was funded by the Defense Advanced Research Projects Agency (DARPA), AD-HELS Program; contract number H0011-06-1-0010. D. Drachenberg acknowledges the support of the Directed Energy Professional Society (DEPS) Graduate Scholarship. NR 26 TC 10 Z9 11 U1 0 U2 20 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1559-128X EI 2155-3165 J9 APPL OPTICS JI Appl. Optics PD OCT 20 PY 2013 VL 52 IS 30 BP 7233 EP 7242 DI 10.1364/AO.52.007233 PG 10 WC Optics SC Optics GA 238EY UT WOS:000325926600004 PM 24216577 ER PT J AU Rahmani, A AF Rahmani, Armin TI QUANTUM DYNAMICS WITH AN ENSEMBLE OF HAMILTONIANS SO MODERN PHYSICS LETTERS B LA English DT Review DE Nonequilibrium dynamics; optimal control; many-body localization; noise ID BOSE-EINSTEIN CONDENSATE; SYSTEMS; GASES; THERMALIZATION; MECHANICS; LATTICES; PHYSICS; STATES AB We review recent progress in the nonequilibrium dynamics of thermally isolated many-body quantum systems, evolving with an ensemble of Hamiltonians as opposed to deterministic evolution with a single time-dependent Hamiltonian. Such questions arise in (i) quantum dynamics of disordered systems, where different realizations of disorder give rise to an ensemble of real-time quantum evolutions, (ii) quantum evolution with noisy Hamiltonians (temporal disorder), which leads to stochastic Schrodinger equations, and, (iii) in the broader context of quantum optimal control, where one needs to analyze an ensemble of permissible protocols in order to find one that optimizes a given figure of merit. The theme of ensemble quantum evolution appears in several emerging new directions in noneqilibrium quantum dynamics of thermally isolated many-body systems, which include many-body localization, noise-driven systems, and shortcuts to adiabaticity. C1 [Rahmani, Armin] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Rahmani, Armin] Los Alamos Natl Lab, CNLS, Los Alamos, NM 87545 USA. RP Rahmani, A (reprint author), Los Alamos Natl Lab, Div Theoret, T-4, Los Alamos, NM 87545 USA. EM armin@lanl.gov FU U.S. Department of Energy under the LANL/LDRD program FX I am grateful to Claudio Chamon, Luca D'Alessio, Eugene Demler, and Takuya Kitagawa for collaboration in research reviewed in this article. I thank Ehud Altman for his careful reading of the manuscript and several helpful suggestions, and David Huse for important comments and discussions. This work was supported by the U.S. Department of Energy under the LANL/LDRD program. NR 70 TC 2 Z9 2 U1 1 U2 15 PU WORLD SCIENTIFIC PUBL CO PTE LTD PI SINGAPORE PA 5 TOH TUCK LINK, SINGAPORE 596224, SINGAPORE SN 0217-9849 EI 1793-6640 J9 MOD PHYS LETT B JI Mod. Phys. Lett. B PD OCT 20 PY 2013 VL 27 IS 26 AR 1330019 DI 10.1142/S0217984913300196 PG 22 WC Physics, Applied; Physics, Condensed Matter; Physics, Mathematical SC Physics GA 235LJ UT WOS:000325720100001 ER PT J AU Geach, JE Hickox, RC Bleem, LE Brodwin, M Holder, GP Aird, KA Benson, BA Bhattacharya, S Carlstrom, JE Chang, CL Cho, HM Crawford, TM Crites, AT de Haan, T Dobbs, MA Dudley, J George, EM Hainline, KN Halverson, NW Holzapfel, WL Hoover, S Hou, Z Hrubes, JD Keisler, R Knox, L Lee, AT Leitch, EM Lueker, M Luong-Van, D Marrone, DP McMahon, JJ Mehl, J Meyer, SS Millea, M Mohr, JJ Montroy, TE Myers, AD Padin, S Plagge, T Pryke, C Reichardt, CL Ruhl, JE Sayre, JT Schaffer, KK Shaw, L Shirokoff, E Spieler, HG Staniszewski, Z Stark, AA Story, KT van Engelen, A Vanderlinde, K Vieira, JD Williamson, R Zahn, O AF Geach, J. E. Hickox, R. C. Bleem, L. E. Brodwin, M. Holder, G. P. Aird, K. A. Benson, B. A. Bhattacharya, S. Carlstrom, J. E. Chang, C. L. Cho, H. -M. Crawford, T. M. Crites, A. T. de Haan, T. Dobbs, M. A. Dudley, J. George, E. M. Hainline, K. N. Halverson, N. W. Holzapfel, W. L. Hoover, S. Hou, Z. Hrubes, J. D. Keisler, R. Knox, L. Lee, A. T. Leitch, E. M. Lueker, M. Luong-Van, D. Marrone, D. P. McMahon, J. J. Mehl, J. Meyer, S. S. Millea, M. Mohr, J. J. Montroy, T. E. Myers, A. D. Padin, S. Plagge, T. Pryke, C. Reichardt, C. L. Ruhl, J. E. Sayre, J. T. Schaffer, K. K. Shaw, L. Shirokoff, E. Spieler, H. G. Staniszewski, Z. Stark, A. A. Story, K. T. van Engelen, A. Vanderlinde, K. Vieira, J. D. Williamson, R. Zahn, O. TI A DIRECT MEASUREMENT OF THE LINEAR BIAS OF MID-INFRARED-SELECTED QUASARS AT z approximate to 1 USING COSMIC MICROWAVE BACKGROUND LENSING SO ASTROPHYSICAL JOURNAL LETTERS LA English DT Article DE cosmology: observations ID ACTIVE GALACTIC NUCLEI; SOUTH-POLE TELESCOPE; DIGITAL SKY SURVEY; BOOTES FIELD; DARK-MATTER; MIDINFRARED SELECTION; LUMINOSITY FUNCTION; BLACK-HOLES; GALAXIES; EVOLUTION AB We measure the cross-power spectrum of the projected mass density as traced by the convergence of the cosmic microwave background lensing field from the South Pole Telescope (SPT) and a sample of Type 1 and 2 (unobscured and obscured) quasars at < z > similar to 1 selected with the Wide-field Infrared Survey Explorer, over 2500 deg(2). The cross-power spectrum is detected at approximate to 7 sigma, and we measure a linear bias b = 1.61 +/- 0.22, consistent with clustering analyses. Using an independent lensing map, derived from Planck observations, to measure the cross-spectrum, we find excellent agreement with the SPT analysis. The bias of the combined sample of Type 1 and 2 quasars determined in this work is similar to that previously determined for Type 1 quasars alone; we conclude that obscured and unobscured quasars trace the matter field in a similar way. This result has implications for our understanding of quasar unification and evolution schemes. C1 [Geach, J. E.] Univ Hertfordshire, Ctr Astrophys Res, Sci & Technol Res Inst, Hatfield AL10 9AB, Herts, England. [Geach, J. E.; Holder, G. P.; de Haan, T.; Dobbs, M. A.; Dudley, J.; van Engelen, A.; Vanderlinde, K.] McGill Univ, Dept Phys, Montreal, PQ H3A 2T8, Canada. [Hickox, R. C.; Hainline, K. N.] Dartmouth Coll, Dept Phys & Astron, Wilder Lab 6127, Hanover, NH 03755 USA. [Bleem, L. E.; Benson, B. A.; Bhattacharya, S.; Carlstrom, J. E.; Chang, C. L.; Crawford, T. M.; Crites, A. T.; Hoover, S.; Mehl, J.; Meyer, S. S.; Padin, S.; Plagge, T.; Schaffer, K. K.; Story, K. T.; Williamson, R.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Bleem, L. E.; Carlstrom, J. E.; Hoover, S.; Keisler, R.; Meyer, S. S.; Story, K. T.] Univ Chicago, Dept Phys, Chicago, IL 60637 USA. [Bleem, L. E.; Bhattacharya, S.; Carlstrom, J. E.] Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60440 USA. [Brodwin, M.] Univ Missouri, Dept Phys & Astron, Kansas City, MO 64110 USA. [Aird, K. A.; Hrubes, J. D.; Luong-Van, D.] Univ Chicago, Chicago, IL 60637 USA. [Benson, B. A.; Carlstrom, J. E.; Chang, C. L.; Meyer, S. S.; Schaffer, K. K.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carlstrom, J. E.; Crawford, T. M.; Crites, A. T.; Meyer, S. S.; Padin, S.; Plagge, T.; Williamson, R.] Univ Chicago, Dept Astron & Astrophys, Chicago, IL 60637 USA. [Cho, H. -M.] NIST Quantum Devices Grp, Boulder, CO 80305 USA. [George, E. M.; Holzapfel, W. L.; Lee, A. T.; Shirokoff, E.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Halverson, N. W.] Univ Colorado, Dept Astrophys & Planetary Sci, Boulder, CO 80309 USA. [Halverson, N. W.] Univ Colorado, Dept Phys, Boulder, CO 80309 USA. [Knox, L.] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. [Lee, A. T.; Spieler, H. G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Lueker, M.; Padin, S.; Vieira, J. D.] CALTECH, Pasadena, CA 91125 USA. [Marrone, D. P.] Univ Arizona, Steward Observ, Tucson, AZ 85721 USA. [McMahon, J. J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Mohr, J. J.] Univ Munich, Dept Phys, D-81679 Munich, Germany. [Mohr, J. J.] Excellence Cluster Univ, D-85748 Garching, Germany. [Mohr, J. J.] Max Planck Inst Extraterr Phys, D-85748 Garching, Germany. [Montroy, T. E.; Sayre, J. T.; Staniszewski, Z.] Case Western Reserve Univ, Dept Phys, Ctr Educ & Res Cosmol & Astrophys, Cleveland, OH 44106 USA. [Myers, A. D.] Univ Wyoming, Dept Phys & Astron, Laramie, WY 82072 USA. [Pryke, C.] Univ Minnesota, Dept Phys, Minneapolis, MN 55455 USA. [Schaffer, K. K.] Sch Art Inst Chicago, Liberal Arts Dept, Chicago, IL 60603 USA. [Stark, A. A.] Harvard Smithsonian Ctr Astrophys, Cambridge, MA 02138 USA. [Vanderlinde, K.] Univ Toronto, Dunlap Inst Astron & Astrophys, Toronto, ON M5S 3H4, Canada. [Vanderlinde, K.] Univ Toronto, Dept Astron & Astrophys, Toronto, ON M5S 3H4, Canada. [Zahn, O.] Univ Calif Berkeley, Berkeley Ctr Cosmol Phys, Dept Phys, Berkeley, CA 94720 USA. RP Geach, JE (reprint author), Univ Hertfordshire, Ctr Astrophys Res, Sci & Technol Res Inst, Hatfield AL10 9AB, Herts, England. EM j.geach@herts.ac.uk RI Williamson, Ross/H-1734-2015; Holzapfel, William/I-4836-2015; OI Williamson, Ross/0000-0002-6945-2975; Aird, Kenneth/0000-0003-1441-9518; Reichardt, Christian/0000-0003-2226-9169; Stark, Antony/0000-0002-2718-9996 FU NSF [ANT-0638937, ANT-0130612, 1211096, 1211112, PHYS-1066293]; NSF Physics Frontier Center [PHY-0114422]; Kavli Foundation; Gordon and Betty Moore Foundation; NASA through ADAP [NNX12AE38G]; NSERC; CIfAR; Canada Research Chairs program; Office of Science of the U.S. DoE [DE-AC02-05CH11231]; ESA Member States; NASA FX SPT is supported by the NSF through grants ANT-0638937 and ANT-0130612. Support for this work is provided by: the NSF Physics Frontier Center grant PHY-0114422 to the Kavli Institute of Cosmological Physics at the University of Chicago; the Kavli Foundation and the Gordon and Betty Moore Foundation; NSF (grant numbers 1211096, 1211112 and PHYS-1066293); NASA through ADAP award NNX12AE38G; NSERC, CIfAR, and the Canada Research Chairs program. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. DoE under contract DE-AC02-05CH11231. Research at Argonne National Laboratory is supported by the Office of Science of the U.S. DoE under contract DE-AC02-06CH11357. Planck is an ESA science mission with instruments and contributions directly funded by ESA Member States, NASA, and Canada. NR 38 TC 26 Z9 26 U1 1 U2 8 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 2041-8205 EI 2041-8213 J9 ASTROPHYS J LETT JI Astrophys. J. Lett. PD OCT 20 PY 2013 VL 776 IS 2 AR L41 DI 10.1088/2041-8205/776/2/L41 PG 6 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 232JO UT WOS:000325490200024 ER PT J AU Singer, LP Cenko, SB Kasliwal, MM Perley, DA Ofek, EO Brown, DA Nugent, PE Kulkarni, SR Corsi, A Frail, DA Bellm, E Mulchaey, J Arcavi, I Barlow, T Bloom, JS Cao, Y Gehrels, N Horesh, A Masci, FJ McEnery, J Rau, A Surace, JA Yaron, O AF Singer, Leo P. Cenko, S. Bradley Kasliwal, Mansi M. Perley, Daniel A. Ofek, Eran O. Brown, Duncan A. Nugent, Peter E. Kulkarni, S. R. Corsi, Alessandra Frail, Dale A. Bellm, Eric Mulchaey, John Arcavi, Iair Barlow, Tom Bloom, Joshua S. Cao, Yi Gehrels, Neil Horesh, Assaf Masci, Frank J. McEnery, Julie Rau, Arne Surace, Jason A. Yaron, Ofer TI DISCOVERY AND REDSHIFT OF AN OPTICAL AFTERGLOW IN 71 deg(2): iPTF13bxl AND GRB 130702A SO ASTROPHYSICAL JOURNAL LETTERS LA English DT Article DE gamma-ray burst: individual (GRB 130702A) ID GAMMA-RAY BURST; 28 FEBRUARY 1997; LIGHT CURVES; ERROR BOX; SUPERNOVA; SWIFT; REPOSITORY; TELESCOPE; SPECTRA; MISSION AB We report the discovery of the optical afterglow of the gamma-ray burst (GRB) 130702A, identified upon searching 71 deg(2) surrounding the Fermi Gamma-ray Burst Monitor (GBM) localization. Discovered and characterized by the intermediate Palomar Transient Factory, iPTF13bxl is the first afterglow discovered solely based on a GBM localization. Real-time image subtraction, machine learning, human vetting, and rapid response multi-wavelength follow-up enabled us to quickly narrow a list of 27,004 optical transient candidates to a single afterglow-like source. Detection of a new, fading X-ray source by Swift and a radio counterpart by CARMA and the Very Large Array confirmed the association between iPTF13bxl and GRB 130702A. Spectroscopy with the Magellan and Palomar 200 inch telescopes showed the afterglow to be at a redshift of z = 0.145, placing GRB 130702A among the lowest redshift GRBs detected to date. The prompt gamma-ray energy release and afterglow luminosity are intermediate between typical cosmological GRBs and nearby sub-luminous events such as GRB 980425 and GRB 060218. The bright afterglow and emerging supernova offer an opportunity for extensive panchromatic follow-up. Our discovery of iPTF13bxl demonstrates the first observational proof-of-principle for similar to 10 Fermi-iPTF localizations annually. Furthermore, it represents an important step toward overcoming the challenges inherent in uncovering faint optical counterparts to comparably localized gravitational wave events in the Advanced LIGO and Virgo era. C1 [Singer, Leo P.; Brown, Duncan A.] CALTECH, LIGO Lab, Pasadena, CA 91125 USA. [Cenko, S. Bradley; Gehrels, Neil; McEnery, Julie] NASA, Goddard Space Flight Ctr, Astrophys Sci Div, Greenbelt, MD 20771 USA. [Kasliwal, Mansi M.; Mulchaey, John] Observ Carnegie Inst Sci, Pasadena, CA 91101 USA. [Perley, Daniel A.; Kulkarni, S. R.; Bellm, Eric; Barlow, Tom; Cao, Yi; Horesh, Assaf] CALTECH, Cahill Ctr Astrophys, Pasadena, CA 91125 USA. [Ofek, Eran O.; Arcavi, Iair; Yaron, Ofer] Weizmann Inst Sci, Benoziyo Ctr Astrophys, IL-76100 Rehovot, Israel. [Brown, Duncan A.] Syracuse Univ, Dept Phys, Syracuse, NY 13244 USA. [Nugent, Peter E.; Bloom, Joshua S.] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. [Nugent, Peter E.; Bloom, Joshua S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Corsi, Alessandra] George Washington Univ, Washington, DC 20052 USA. [Frail, Dale A.] Natl Radio Astron Observ, Socorro, NM 87801 USA. [Masci, Frank J.; Surace, Jason A.] CALTECH, Infrared Proc & Anal Ctr, Pasadena, CA 91125 USA. [Rau, Arne] Max Planck Inst Extraterr Phys, D-85748 Garching, Germany. RP Singer, LP (reprint author), CALTECH, LIGO Lab, Pasadena, CA 91125 USA. EM lsinger@caltech.edu RI Horesh, Assaf/O-9873-2016; OI Horesh, Assaf/0000-0002-5936-1156; Singer, Leo/0000-0001-9898-5597 FU National Science Foundation [PHY-0847611]; NSF-CDI grant [0941742]; Carnegie-Princeton Fellowship; NASA through the Hubble Fellowship [HST-HF-51293.01, HST-HF-51296.01-A]; Space Telescope Science Institute; NASA [NAS 5-26555]; Israeli Ministry of Science; I-CORE Program; RCSA Cottrell Scholar award FX This research is supported by the National Science Foundation through a Graduate Research Fellowship for L. P. S., award PHY-0847611 for D. A. B., and NSF-CDI grant 0941742 for J.S.B. M. M. K. acknowledges generous support from the Carnegie-Princeton Fellowship. M. M. K. and D. A. P. are supported by NASA through the Hubble Fellowship grants HST-HF-51293.01 and HST-HF-51296.01-A, awarded by the Space Telescope Science Institute, which is operated by the Association of Universities for Research in Astronomy, Inc., for NASA, under contract NAS 5-26555. E.O.O. is the incumbent of the Arye Dissentshik career development chair and is supported by grants from the Israeli Ministry of Science and the I-CORE Program. D. A. B. is further supported by an RCSA Cottrell Scholar award. NR 39 TC 22 Z9 24 U1 0 U2 3 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 2041-8205 J9 ASTROPHYS J LETT JI Astrophys. J. Lett. PD OCT 20 PY 2013 VL 776 IS 2 AR L34 DI 10.1088/2041-8205/776/2/L34 PG 7 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 232JO UT WOS:000325490200017 ER PT J AU Shen, YF Liu, YD Sun, X Wang, YD Zuo, L Misra, RDK AF Shen, Y. F. Liu, Y. D. Sun, X. Wang, Y. D. Zuo, L. Misra, R. D. K. TI Improved ductility of a transformation-induced-plasticity steel by nanoscale austenite lamellae SO MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING LA English DT Article DE TRIP steel; Retained austenite; Nanoscale lamellae; Mechanical properties ID ASSISTED MULTIPHASE STEELS; PLAIN CARBON-STEELS; RETAINED AUSTENITE; MARTENSITE-TRANSFORMATION; LATTICE-PARAMETERS; TRIP STEELS; IRON-CARBON; STABILITY; MICROSTRUCTURE; TOUGHNESS AB TRIP (transformation-induced-plasticity) steel with a chemical composition of 0.19C-0.30Si-1.76Mn-1.52Al (weight percentage, wt%) have been treated by intercritical annealing and austempering process. The microstructures of the obtained samples consist of the ferrite, the bainite and the retained austenite phase. The volume fractions of the bainite and the retained austenite gradually increase with increasing the temperature of the intercritical annealing. Consequently, significantly different mechanical properties have been observed. The sample annealed at 820 degrees C (for 120 s) and partitioned at 400 degrees C (for 300 s) has the best combination of ultimate tensile strength (UTS, similar to 682 MPa) and elongation to failure (similar to 70%) with about 26% of bainitic ferrite plates and 17% retained austenite in its microstructure. The retained austenite has a lamella morphology with 100-300 nm in thickness and 2-5 mu m in length. On the contrary, the sample annealed at the same temperature without the partitioning process yields much lower UTS and elongation to failure. (c) 2013 Elsevier B.V. All rights reserved. C1 [Shen, Y. F.; Liu, Y. D.; Wang, Y. D.; Zuo, L.] Northeastern Univ, Sch Met & Mat, Key Lab Anisotropy & Texture Mat MOE, Shenyang 110004, Peoples R China. [Sun, X.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Misra, R. D. K.] Univ Louisiana Lafayette, Inst Mat Res & Innovat, Ctr Struct & Funct Mat, Lab Excellence Adv Steel Res, Lafayette, LA 70504 USA. RP Shen, YF (reprint author), Northeastern Univ, Sch Met & Mat, Key Lab Anisotropy & Texture Mat MOE, Shenyang 110004, Peoples R China. EM shenyf@smm.neu.edu.cn RI wang, yandong/G-9404-2013 FU National Natural Science Foundation of China [51231002]; National Science and Technology Support Project [2011BAE13B03]; Fundamental Research Funds for the Central Universities [N100702001]; Open Program of the State Key Lab of Rolling Automation [N2012001]; US Department of Energy [DE-AC05-76RL01830]; Department of Energy Office of FreedomCar and Vehicle Technologies under the Automotive Lightweighting Materials Program FX This research has been supported by the National Natural Science Foundation of China (Grant no. 51231002), the National Science and Technology Support Project (2011BAE13B03), the Fundamental Research Funds for the Central Universities (N100702001), and the Open Program of the State Key Lab of Rolling & Automation (N2012001). Pacific Northwest National Laboratory (PNNL) is operated by Battelle Memorial Institute for the US Department of Energy under Contract no. DE-AC05-76RL01830. PNNL contribution to this work was funded by the Department of Energy Office of FreedomCar and Vehicle Technologies under the Automotive Lightweighting Materials Program managed by Mr. William Joost. NR 32 TC 10 Z9 11 U1 1 U2 28 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0921-5093 J9 MAT SCI ENG A-STRUCT JI Mater. Sci. Eng. A-Struct. Mater. Prop. Microstruct. Process. PD OCT 20 PY 2013 VL 583 BP 1 EP 10 DI 10.1016/j.msea.2013.06.062 PG 10 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA 210UP UT WOS:000323860500001 ER PT J AU Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, C Rohringer, H Schofbeck, R Strauss, J Taurok, A Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, M Bansal, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Luyckx, S Mucibello, L Ochesanu, S Roland, B Rougny, R Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Kalogeropoulos, A Keaveney, J Maes, M Olbrechts, A Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Clerbaux, B De Lentdecker, G Favart, L Gay, APR Hreus, T Leonard, A Marage, PE Mohammadi, A Reis, T Thomas, L Vander Velde, C Vanlaer, P Wang, J Adler, V Beernaert, K Benucci, L Cimmino, A Costantini, S Dildick, S Garcia, G Klein, B Lellouch, J Marinov, A Mccartin, J Rios, AAO Ryckbosch, D Sigamani, M Strobbe, N Thyssen, F Tytgat, M Walsh, S Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bruno, G Castello, R Caudron, A Ceard, L Delaere, C du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Lemaitre, V Liao, J Militaru, O Nuttens, C Pagano, D Pin, A Piotrzkowski, K Popov, A Selvaggi, M Garcia, JMV Beliy, N Caebergs, T Daubie, E Hammad, GH Alves, GA Martins, MC Martins, T Pol, ME Souza, MHG Alda, WL Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD De Souza, SF Malbouisson, H Malek, M Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santoro, A Jorge, LS Sznajder, A Manganote, EJT Pereira, AV Anjos, TS Bernardes, CA Dias, FA Tomei, TRFP Gregores, EM Lagana, C Marinho, F Mercadante, PG Novaes, SF Padula, SS Genchev, V Iaydjiev, P Piperov, S Rodozov, M Stoykova, S Sultanov, G Tcholakov, V Trayanov, R Vutova, M Dimitrov, A Hadjiiska, R Kozhuharov, V Litov, L Pavlov, B Petkov, P Bian, JG Chen, GM Chen, HS Jiang, CH Liang, D Liang, S Meng, X Tao, J Wang, J Wang, X Wang, Z Xiao, H Xu, M Asawatangtrakuldee, C Ban, Y Guo, Y Li, Q Li, W Liu, S Mao, Y Qian, SJ Wang, D Zhang, L Zou, W Avila, C Montoya, CAC Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Plestina, R Polic, D Puljak, I Antunovic, Z Kovac, M Brigljevic, V Duric, S Kadija, K Luetic, J Mekterovic, D Morovic, S Tikvica, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Finger, M Finger, M Assran, Y Kamel, AE Mahmoud, MA Mahrous, A Radi, A Kadastik, M Muntel, M Murumaa, M Raidal, M Rebane, L Tiko, A Eerola, P Fedi, G Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Kortelainen, MJ Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E Wendland, L Korpela, A Tuuva, T Besancon, M Choudhury, S Couderc, F Dejardin, M Denegri, D Fabbro, B Faure, JL Ferri, F Ganjour, S Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Malcles, J Millischer, L Nayak, A Rander, J Rosowsky, A Titov, M Baffioni, S Beaudette, F Benhabib, L Bianchini, L Bluj, M Busson, P Charlot, C Daci, N Dahms, T Dalchenko, M Dobrzynski, L Florent, A de Cassagnac, RG Haguenauer, M Mine, P Mironov, C Naranjo, IN Nguyen, M Ochando, C Paganini, P Sabes, D Salerno, R Sirois, Y Veelken, C Zabi, A Agram, JL Andrea, J Bloch, D Bodin, D Brom, JM Chabert, EC Collard, C Conte, E Drouhin, F Fontaine, JC Gele, D Goerlach, U Goetzmann, C Juillot, P Le Bihan, AC Van Hove, P Beauceron, S Beaupere, N Boudoul, G Brochet, S Chasserat, J Chierici, R Contardo, D Depasse, P El Mamouni, H Fay, J Gascon, S Gouzevitch, M Ille, B Kurca, T Lethuillier, M Mirabito, L Perries, S Sgandurra, L Sordini, V Tschudi, Y Vander Donckt, M Verdier, P Viret, S Tsamalaidze, Z Autermann, C Beranek, S Calpas, B Edelhoff, M Feld, L Heracleous, N Hindrichs, O Klein, K Merz, J Ostapchuk, A Perieanu, A Raupach, F Sammet, J Schael, S Sprenger, D Weber, H Wittmer, B Zhukov, V Ata, M Caudron, J Dietz-Laursonn, E Duchardt, D Erdmann, M Fischer, R Guth, A Hebbeker, T Heidemann, C Hoepfner, K Klingebiel, D Kreuzer, P Merschmeyer, M Meyer, A Olschewski, M Padeken, K Papacz, P Pieta, H Reithler, H Schmitz, SA Sonnenschein, L Steggemann, J Teyssier, D Thuer, S Weber, M Cherepanov, V Erdogan, Y Flugge, G Geenen, H Geisler, M Ahmad, WH Hoehle, F Kargoll, B Kress, T Kuessel, Y Lingemann, J Nowack, A Nugent, IM Perchalla, L Pooth, O Stahl, A Martin, MA Asin, I Bartosik, N Behr, J Behrenhoff, W Behrens, U Bergholz, M Bethani, A Borras, K Burgmeier, A Cakir, A Calligaris, L Campbell, A Costanza, F Pardos, CD Dorland, T Eckerlin, G Eckstein, D Flucke, G Geiser, A Glushkov, I Gunnellini, P Habib, S Hauk, J Hellwig, G Jung, H Kasemann, M Katsas, P Kleinwort, C Kluge, H Kramer, M Krucker, D Kuznetsova, E Lange, W Leonard, J Lipka, K Lohmann, W Lutz, B Mankel, R Marfin, I Melzer-Pellmann, IA Meyer, AB Mnich, J Mussgiller, A Naumann-Emme, S Novgorodova, O Nowak, F Olzem, J Perrey, H Petrukhin, A Pitzl, D Raspereza, A Cipriano, PMR Riedl, C Ron, E Salfeld-Nebgen, J Schmidt, R Schoerner-Sadenius, T Sen, N Stein, M Walsh, R Wissing, C Blobel, V Enderle, H Erfle, J Gebbert, U Gorner, M Gosselink, M Haller, J Heine, K Hoing, RS Kaussen, G Kirschenmann, H Klanner, R Lange, J Peiffer, T Pietsch, N Rathjens, D Sander, C Schettler, H Schleper, P Schlieckau, E Schmidt, A Schroder, M Schum, T Seidel, M Sibille, J Sola, V Stadie, H Steinbruck, G Thomsen, J Vanelderen, L Barth, C Baus, C Berger, J Boser, C Chwalek, T De Boer, W Descroix, A Dierlamm, A Feindt, M Guthoff, M Hackstein, C Hartmann, F Hauth, T Heinrich, M Held, H Hoffmann, KH Husemann, U 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CA CMS Collaboration TI Measurement of the ratio of the inclusive 3-jet cross section to the inclusive 2-jet cross section in pp collisions at root s=7 TeV and first determination of the strong coupling constant in the TeV range SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID SMALL-DISTANCE-BEHAVIOUR; PARTON DISTRIBUTIONS; FIELD THEORY; LHC AB A measurement is presented of the ratio of the inclusive 3-jet cross section to the inclusive 2-jet cross section as a function of the average transverse momentum, < p(T1,2)>, of the two leading jets in the event. The data sample was collected during 2011 at a proton-proton centre-of-mass energy of 7 TeV with the CMS detector at the LHC, corresponding to an integrated luminosity of 5.0 fb(-1). The strong coupling constant at the scale of the Z boson mass is determined to be alpha(S)(M-Z) = 0.1148 +/- 0.0014 (exp.) +/- 0.0018 (PDF) +/- 0.0050 (theory), by comparing the ratio in the range 0.42 < < p(T1,2)> < 1.39 TeV to the predictions of perturbative QCD at next-to-leading order. This is the first determination of alpha(S)(M-Z) from measurements at momentum scales beyond 0.6 TeV. The predicted ratio depends only indirectly on the evolution of the parton distribution functions of the proton such that this measurement also serves as a test of the evolution of the strong coupling constant. No deviation from the expected behaviour is observed. C1 [Chatrchyan, S.; Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Bergauer, T.; Dragicevic, M.; Eroe, J.; Fabjan, C.; Friedl, M.; Fruehwirth, R.; Ghete, V. M.; Hoermann, N.; Hrubec, J.; Jeitler, M.; Kiesenhofer, W.; Knuenz, V.; Krammer, M.; Kraetschmer, I.; Liko, D.; Mikulec, I.; Rabady, D.; Rahbaran, B.; Rohringer, C.; Rohringer, H.; Schoefbeck, R.; Strauss, J.; Taurok, A.; Treberer-Treberspurg, W.; Waltenberger, W.; Wulz, C. -E.] OeAW, Inst Hochenergiephys, Vienna, Austria. [Mossolov, V.; Shumeiko, N.; Gonzalez, J. Suarez] Natl Ctr Particle & High Energy Phys, Minsk, Byelarus. [Alderweireldt, S.; Bansal, M.; Bansal, S.; Cornelis, T.; De Wolf, E. A.; Janssen, X.; Knutsson, A.; Luyckx, S.; Mucibello, L.; Ochesanu, S.; Roland, B.; Rougny, R.; Van Haevermaet, H.; Van Mechelen, P.; Van Remortel, N.; Van Spilbeeck, A.] Univ Antwerp, B-2020 Antwerp, Belgium. [Blekman, F.; Blyweert, S.; D'Hondt, J.; Kalogeropoulos, A.; Keaveney, J.; Maes, M.; Olbrechts, A.; Tavernier, S.; Van Doninck, W.; Van Mulders, P.; Van Onsem, G. P.; Villella, I.] Vrije Univ Brussel, Brussels, Belgium. [Clerbaux, B.; De Lentdecker, G.; Favart, L.; Gay, A. P. R.; Hreus, T.; Leonard, A.; Marage, P. E.; Mohammadi, A.; Reis, T.; Thomas, L.; Vander Velde, C.; Vanlaer, P.; Wang, J.] Univ Libre Bruxelles, Brussels, Belgium. [Adler, V.; Beernaert, K.; Benucci, L.; Cimmino, A.; Costantini, S.; Dildick, S.; Garcia, G.; Klein, B.; Lellouch, J.; Marinov, A.; Mccartin, J.; Rios, A. A. Ocampo; Ryckbosch, D.; Sigamani, M.; Strobbe, N.; Thyssen, F.; Tytgat, M.; Walsh, S.; Yazgan, E.; Zaganidis, N.] Univ Ghent, B-9000 Ghent, Belgium. [Basegmez, S.; Beluffi, C.; Bruno, G.; Castello, R.; Caudron, A.; Ceard, L.; Delaere, C.; du Pree, T.; Favart, D.; Forthomme, L.; Giammanco, A.; Hollar, J.; Lemaitre, V.; Liao, J.; Militaru, O.; Nuttens, C.; Pagano, D.; Pin, A.; Piotrzkowski, K.; Popov, A.; Selvaggi, M.; Garcia, J. M. Vizan] Catholic Univ Louvain, B-1348 Louvain, Belgium. [Beliy, N.; Caebergs, T.; Daubie, E.; Hammad, G. H.] Univ Mons, B-7000 Mons, Belgium. [Alves, G. A.; Correa Martins Junior, M.; Martins, T.; Pol, M. E.; Souza, M. H. G.] Ctr Brasileiro Pesquisas Fis, Rio De Janeiro, Brazil. [Alda Junior, W. L.; Carvalho, W.; Chinellato, J.; Custodio, A.; Da Costa, E. M.; De Jesus Damiao, D.; De Oliveira Martins, C.; Fonseca De Souza, S.; Malbouisson, H.; Malek, M.; Matos Figueiredo, D.; Mundim, L.; Nogima, H.; Prado Da Silva, W. L.; Santoro, A.; Soares Jorge, L.; Sznajder, A.; Tonelli Manganote, E. J.; Vilela Pereira, A.] Univ Estado Rio de Janeiro, BR-20550011 Rio De Janeiro, Brazil. [Anjos, T. S.; Bernardes, C. A.; Dias, F. A.; Fernandez Perez Tomei, T. R.; Gregores, E. M.; Lagana, C.; Marinho, F.; Mercadante, P. G.; Novaes, S. F.; Padula, S. S.] Univ Estadual Paulista, Sao Paulo, Brazil. [Genchev, V.; Iaydjiev, P.; Piperov, S.; Rodozov, M.; Stoykova, S.; Sultanov, G.; Tcholakov, V.; Trayanov, R.; Vutova, M.] Bulgarian Acad Sci, Inst Nucl Res & Nucl Energy, Sofia, Bulgaria. [Dimitrov, A.; Hadjiiska, R.; Kozhuharov, V.; Litov, L.; Pavlov, B.; Petkov, P.] Univ Sofia, BU-1126 Sofia, Bulgaria. [Wang, J.; Bian, J. G.; Chen, G. M.; Chen, H. S.; Jiang, C. H.; Liang, D.; Liang, S.; Meng, X.; Tao, J.; Wang, X.; Wang, Z.; Xiao, H.; Xu, M.] Inst High Energy Phys, Beijing 100039, Peoples R China. [Asawatangtrakuldee, C.; Ban, Y.; Guo, Y.; Li, Q.; Li, W.; Liu, S.; Mao, Y.; Qian, S. J.; Wang, D.; Zhang, L.; Zou, W.] Peking Univ, State Key Lab Nucl Phys & Technol, Beijing 100871, Peoples R China. [Avila, C.; Carrillo Montoya, C. A.; Gomez, J. P.; Gomez Moreno, B.; Sanabria, J. C.] Univ Los Andes, Bogota, Colombia. [Godinovic, N.; Lelas, D.; Plestina, R.; Polic, D.; Puljak, I.] Tech Univ Split, Split, Croatia. [Antunovic, Z.; Kovac, M.] Univ Split, Split, Croatia. [Brigljevic, V.; Duric, S.; Kadija, K.; Luetic, J.; Mekterovic, D.; Morovic, S.; Tikvica, L.] Rudjer Boskovic Inst, Zagreb, Croatia. [Attikis, A.; Mavromanolakis, G.; Mousa, J.; Nicolaou, C.; Ptochos, F.; Razis, P. A.] Univ Cyprus, Nicosia, Cyprus. [Finger, M.; Finger, M., Jr.] Charles Univ Prague, Prague, Czech Republic. [Assran, Y.; Kamel, A. Ellithi; Mahmoud, M. A.; Mahrous, A.; Radi, A.] Acad Sci Res & Technol Arab Republ Egypt, Egyptian Network High Energy Phys, Cairo, Egypt. [Kadastik, M.; Muentel, M.; Murumaa, M.; Raidal, M.; Rebane, L.; Tiko, A.] NICPB, Tallinn, Estonia. [Eerola, P.; Fedi, G.; Voutilainen, M.] Univ Helsinki, Dept Phys, Helsinki, Finland. [Harkonen, J.; Karimaki, V.; Kinnunen, R.; Kortelainen, M. J.; Lampen, T.; Lassila-Perini, K.; Lehti, S.; Linden, T.; Luukka, P.; Maenpaa, T.; Peltola, T.; Tuominen, E.; Tuominiemi, J.; Tuovinen, E.; Wendland, L.] Helsinki Inst Phys, Helsinki, Finland. [Korpela, A.; Tuuva, T.] Lappeenranta Univ Technol, Lappeenranta, Finland. [Besancon, M.; Choudhury, S.; Couderc, F.; Dejardin, M.; Denegri, D.; Fabbro, B.; Faure, J. L.; Ferri, F.; Ganjour, S.; Givernaud, A.; Gras, P.; de Monchenault, G. Hamel; Jarry, P.; Locci, E.; Malcles, J.; Millischer, L.; Nayak, A.; Rander, J.; Rosowsky, A.; Titov, M.] CEA Saclay, DSM IRFU, F-91191 Gif Sur Yvette, France. [Baffioni, S.; Beaudette, F.; Benhabib, L.; Bianchini, L.; Bluj, M.; Busson, P.; Charlot, C.; Daci, N.; Dahms, T.; Dalchenko, M.; Dobrzynski, L.; Florent, A.; de Cassagnac, R. Granier; Haguenauer, M.; Mine, P.; Mironov, C.; Naranjo, I. N.; Nguyen, M.; Ochando, C.; Paganini, P.; Sabes, D.; Salerno, R.; Sirois, Y.; Veelken, C.; Zabi, A.] Ecole Polytech, CNRS, IN2P3, Lab Leprince Ringuet, F-91128 Palaiseau, France. [Agram, J. -L.; Andrea, J.; Bloch, D.; Bodin, D.; Brom, J. -M.; Chabert, E. C.; Collard, C.; Conte, E.; Drouhin, F.; Fontaine, J. -C.; Gele, D.; Goerlach, U.; Goetzmann, C.; Juillot, P.; Le Bihan, A. -C.; Van Hove, P.] Univ Haute Alsace Mulhouse, Univ Strasbourg, Inst Pluridisciplinaire Hubert Curien, CNRS IN2P3, Strasbourg, France. [Beauceron, S.; Beaupere, N.; Boudoul, G.; Brochet, S.; Chasserat, J.; Chierici, R.; Contardo, D.; Depasse, P.; El Mamouni, H.; Fay, J.; Gascon, S.; Gouzevitch, M.; Ille, B.; Kurca, T.; Lethuillier, M.; Mirabito, L.; Perries, S.; Sgandurra, L.; Sordini, V.; Tschudi, Y.; Vander Donckt, M.; Verdier, P.; Viret, S.] Univ Lyon 1, CNRS, IN2P3, Inst Phys Nucl Lyon, F-69622 Villeurbanne, France. [Tsamalaidze, Z.] Tbilisi State Univ, Inst High Energy Phys & Informatizat, GE-380086 Tbilisi, Rep of Georgia. [Autermann, C.; Beranek, S.; Calpas, B.; Edelhoff, M.; Feld, L.; Heracleous, N.; Hindrichs, O.; Klein, K.; Merz, J.; Ostapchuk, A.; Perieanu, A.; Raupach, F.; Sammet, J.; Schael, S.; Sprenger, D.; Weber, H.; Wittmer, B.; Zhukov, V.] Rhein Westfal TH Aachen, Inst Phys 1, Aachen, Germany. [Ata, M.; Caudron, J.; Dietz-Laursonn, E.; Duchardt, D.; Erdmann, M.; Fischer, R.; Gueth, A.; Hebbeker, T.; Heidemann, C.; Hoepfner, K.; Klingebiel, D.; Kreuzer, P.; Merschmeyer, M.; Meyer, A.; Olschewski, M.; Padeken, K.; Papacz, P.; Pieta, H.; Reithler, H.; Schmitz, S. A.; Sonnenschein, L.; Steggemann, J.; Teyssier, D.; Thueer, S.; Weber, M.] Rhein Westfal TH Aachen, Phys Inst A3, Aachen, Germany. [Cherepanov, V.; Erdogan, Y.; Fluegge, G.; Geenen, H.; Geisler, M.; Ahmad, W. Haj; Hoehle, F.; Kargoll, B.; Kress, T.; Kuessel, Y.; Lingemann, J.; Nowack, A.; Nugent, I. M.; Perchalla, L.; Pooth, O.; Stahl, A.] Rhein Westfal TH Aachen, Phys Inst B3, Aachen, Germany. [Martin, M. Aldaya; Asin, I.; Bartosik, N.; Behr, J.; Behrenhoff, W.; Behrens, U.; Bergholz, M.; Bethani, A.; Borras, K.; Burgmeier, A.; Cakir, A.; Calligaris, L.; Campbell, A.; Costanza, F.; Pardos, C. Diez; Dorland, T.; Eckerlin, G.; Eckstein, D.; Flucke, G.; Geiser, A.; Glushkov, I.; Gunnellini, P.; Habib, S.; Hauk, J.; Hellwig, G.; Jung, H.; Kasemann, M.; Katsas, P.; Kleinwort, C.; Kluge, H.; Kraemer, M.; Kruecker, D.; Kuznetsova, E.; Lange, W.; Leonard, J.; Lipka, K.; Lohmann, W.; Lutz, B.; Mankel, R.; Marfin, I.; Melzer-Pellmann, I. -A.; Meyer, A. B.; Mnich, J.; Mussgiller, A.; Naumann-Emme, S.; Novgorodova, O.; Nowak, F.; Olzem, J.; Perrey, H.; Petrukhin, A.; Pitzl, D.; Raspereza, A.; Cipriano, P. M. Ribeiro; Riedl, C.; Ron, E.; Salfeld-Nebgen, J.; Schmidt, R.; Schoerner-Sadenius, T.; Sen, N.; Stein, M.; Walsh, R.; Wissing, C.] DESY, Hamburg, Germany. [Blobel, V.; Enderle, H.; Erfle, J.; Gebbert, U.; Goerner, M.; Gosselink, M.; Haller, J.; Heine, K.; Hoeing, R. S.; Kaussen, G.; Kirschenmann, H.; Klanner, R.; Lange, J.; Peiffer, T.; Pietsch, N.; Rathjens, D.; Sander, C.; Schettler, H.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Schroeder, M.; Schum, T.; Seidel, M.; Sibille, J.; Sola, V.; Stadie, H.; Steinbrueck, G.; Thomsen, J.; Vanelderen, L.] Univ Hamburg, Hamburg, Germany. [Barth, C.; Baus, C.; Berger, J.; Boeser, C.; Chwalek, T.; De Boer, W.; Descroix, A.; Dierlamm, A.; Feindt, M.; Guthoff, M.; Hackstein, C.; Hartmann, F.; Hauth, T.; Heinrich, M.; Held, H.; Hoffmann, K. H.; Husemann, U.; Katkov, I.; Komaragiri, J. R.; Kornmayer, A.; Pardo, P. Lobelle; Martschei, D.; Mueller, S.; Mueller, Th.; Niegel, M.; Nuernberg, A.; Oberst, O.; Ott, J.; Quast, G.; Rabbertz, K.; Ratnikov, F.; Ratnikova, N.; Roecker, S.; Schilling, F. -P.; Schott, G.; Simonis, H. J.; Stober, F. M.; Troendle, D.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weiler, T.; Zeise, M.] Univ Karlsruhe, Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Kesisoglou, S.; Kyriakis, A.; Loukas, D.; Markou, A.; Markou, C.; Ntomari, E.] NCSR Demokritos, INPP, Aghia Paraskevi, Greece. [Gouskos, L.; Mertzimekis, T. J.; Panagiotou, A.; Saoulidou, N.; Stiliaris, E.] Univ Athens, Athens, Greece. [Aslanoglou, X.; Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Manthos, N.; Papadopoulos, I.; Paradas, E.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hidas, P.; Horvath, D.; Radics, B.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.] KFKI Res Inst Particle & Nucl Phys, Budapest, Hungary. [Beni, N.; Czellar, S.; Molnar, J.; Palinkas, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Karancsi, J.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, H-4012 Debrecen, Hungary. [Beri, S. B.; Bhatnagar, V.; Dhingra, N.; Gupta, R.; Kaur, M.; Mehta, M. Z.; Mittal, M.; Nishu, N.; Saini, L. K.; Sharma, A.; Singh, J. B.] Panjab Univ, Chandigarh 160014, India. [Kumar, Ashok; Kumar, Arun; Ahuja, S.; Bhardwaj, A.; Choudhary, B. C.; Malhotra, S.; Naimuddin, M.; Ranjan, K.; Saxena, P.; Sharma, V.; Shivpuri, R. K.] Univ Delhi, Delhi 110007, India. [Banerjee, S.; Bhattacharya, S.; Chatterjee, K.; Dutta, S.; Gomber, B.; Jain, Sa.; Jain, Sh.; Khurana, R.; Modak, A.; Mukherjee, S.; Roy, D.; Sarkar, S.; Sharan, M.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Dutta, D.; Kailas, S.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Bombay 400085, Maharashtra, India. [Aziz, T.; Chatterjee, R. M.; Ganguly, S.; Guchait, M.; Gurtu, A.; Maity, M.; Majumder, G.; Mazumdar, K.; Mohanty, G. B.; Parida, B.; Sudhakar, K.; Wickramage, N.] Tata Inst Fundamental Res EHEP, Bombay, Maharashtra, India. [Banerjee, S.; Dugad, S.] Tata Inst Fundamental Res HECR, Bombay, Maharashtra, India. [Arfaei, H.; Bakhshiansohi, H.; Etesami, S. M.; Fahim, A.; Hesari, H.; Jafari, A.; Khakzad, M.; Najafabadi, M. Mohammadi; Mehdiabadi, S. Paktinat; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; Colaleo, A.; Creanza, D.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; Marangelli, B.; My, S.; Nuzzo, S.; Pacifico, N.; Pompili, A.; Pugliese, G.; Selvaggi, G.; Silvestris, L.; Singh, G.; Venditti, R.; Verwilligen, P.; Zito, G.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; De Palma, M.; Marangelli, B.; Nuzzo, S.; Pompili, A.; Selvaggi, G.; Singh, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Meneghelli, M.; Montanari, A.; Navarria, F. L.; Odorici, F.; Perrotta, A.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Meneghelli, M.; Navarria, F. L.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Albergo, S.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Albergo, S.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gallo, E.; Gonzi, S.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gonzi, S.; Lenzi, P.; Tropiano, A.] Univ Florence, Florence, Italy. [Fabbri, F.; Benussi, L.; Bianco, S.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Fabbricatore, P.; Musenich, R.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Tosi, S.] Univ Genoa, Genoa, Italy. [Benaglia, A.; De Guio, F.; Di Matteo, L.; Fiorendi, S.; Gennai, S.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Massironi, A.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] Ist Nazl Fis Nucl, Sez Milano Bicocca, I-20133 Milan, Italy. [De Guio, F.; Di Matteo, L.; Fiorendi, S.; Ghezzi, A.; Govoni, P.; Lucchini, M. T.; Manzoni, R. A.; Martelli, A.; Massironi, A.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; De Cosa, A.; Fabozzi, F.; Iorio, A. O. M.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [De Cosa, A.; Iorio, A. O. M.] Univ Naples Federico II, Naples, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata Potenza, Naples, Italy. [Meola, S.] Univ G Marconi Roma, Naples, Italy. [Azzi, P.; Bacchetta, N.; Bellan, P.; Biasotto, M.; Bisello, D.; Branca, A.; Carlin, R.; Checchia, P.; Dorigo, T.; Fanzago, F.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Gonella, F.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Lazzizzera, I.; Margoni, M.; Meneguzzo, A. T.; Montecassiano, F.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Sgaravatto, M.; Simonetto, F.; Torassa, E.; Tosi, M.; Zotto, P.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Bellan, P.; Bisello, D.; Branca, A.; Carlin, R.; Galanti, M.; Gasparini, F.; Gasparini, U.; Giubilato, P.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.] Univ Padua, Padua, Italy. [Kanishchev, K.; Lazzizzera, I.] Univ Trento Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Nappi, A.; Romeo, F.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Biasini, M.; Fano, L.; Lariccia, P.; Mantovani, G.; Nappi, A.; Romeo, F.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Boccali, T.; Broccolo, G.; Castaldi, R.; D'Agnolo, R. T.; Dell'Orso, R.; Fiori, F.; Foa, L.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Vernieri, C.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; D'Agnolo, R. T.; Fiori, F.; Foa, L.; Ligabue, F.; Vernieri, C.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Diemoz, M.; Fanelli, C.; Grassi, M.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Soffi, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; Del Re, D.; Fanelli, C.; Grassi, M.; Longo, E.; Margaroli, F.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Soffi, L.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Biino, C.; Cartiglia, N.; Casasso, S.; Costa, M.; Dellacasa, G.; Demaria, N.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Pastrone, N.; Pelliccioni, M.; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Casasso, S.; Costa, M.; Migliore, E.; Monaco, V.; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Montanino, D.; Penzo, A.; Schizzi, A.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Kim, T. Y.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Chang, S.; Kim, D. H.; Kim, G. N.; Kim, J. E.; Kong, D. J.; Oh, Y. D.; Park, H.; Son, D. C.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, J. Y.; Kim, Z. J.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, T. J.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. S.; Kwon, E.; Lee, B.; Lee, J.; Lee, S.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Grigelionis, I.; Juodagalvis, A.] Vilnius State Univ, Vilnius, Lithuania. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Lopez-Fernandez, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.; Reyes-Santos, M. A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Bell, A. J.; Butler, P. H.; Doesburg, R.; Reucroft, S.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Asghar, M. I.; Butt, J.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Wolszczak, W.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Almeida, N.; Bargassa, P.; David, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Rodrigues Antunes, J.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Kozlov, G.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Evstyukhin, S.; Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Erofeeva, M.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Markina, A.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Ekmedzic, M.; Krpic, D.; Milosevic, J.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Ekmedzic, M.; Krpic, D.; Milosevic, J.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Alcaraz Maestre, J.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Navarro De Martino, E.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.; Willmott, C.] CIEMAT, E-28040 Madrid, Spain. [Albajar, C.; de Troconiz, J. F.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.; Piedra Gomez, J.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Chuang, S. H.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Graziano, A.; Jorda, C.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Sharma, A.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Bendavid, J.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Bondu, O.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Perez, J. A. Coarasa; Colafranceschi, S.; d'Enterria, D.; Dabrowski, A.; De Roeck, A.; De Visscher, S.; Di Guida, S.; Dobson, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Funk, W.; Georgiou, G.; Giffels, M.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Giunta, M.; Glege, F.; Garrido, R. Gomez-Reino; Gowdy, S.; Guida, R.; Hammer, J.; Hansen, M.; Harris, P.; Hartl, C.; Hegner, B.; Hinzmann, A.; Innocente, V.; Janot, P.; Kaadze, K.; Karavakis, E.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lee, Y. -J.; Lourenco, C.; Magini, N.; Malberti, M.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moser, R.; Mulders, M.; Musella, P.; Nesvold, E.; Orsini, L.; Cortezon, E. Palencia; Perez, E.; Perrozzi, L.; Petrilli, A.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Piparo, D.; Polese, G.; Quertenmont, L.; Racz, A.; Reece, W.; Rojo, J.; Rolandi, G.; Rovelli, C.; Rovere, M.; Sakulin, H.; Santanastasio, F.; Schaefer, C.; Schwick, C.; Segoni, I.; Sekmen, S.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Stoye, M.; Tsirou, A.; Veres, G. I.; Vlimant, J. R.; Woehri, H. K.; Worm, S. D.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Gabathuler, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Meier, F.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bortignon, P.; Buchmann, M. A.; Casal, B.; Chanon, N.; Deisher, A.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eller, P.; Grab, C.; Hits, D.; Lecomte, P.; Lustermann, W.; Marini, A. C.; del Arbol, P. Martinez Ruiz; Mohr, N.; Moortgat, F.; Naegeli, C.; Nef, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pape, L.; Peruzzi, M.; Ronga, F. J.; Rossini, M.; Sala, L.; Sanchez, A. K.; Starodumov, A.; Stieger, B.; Takahashi, M.; Tauscher, L.; Thea, A.; Theofilatos, K.; Treille, D.; Urscheler, C.; Wallny, R.; Weber, H. A.] Swiss Fed Inst Technol, Inst Particle Phys, Zurich, Switzerland. [Amsler, C.; Chiochia, V.; Favaro, C.; Rikova, M. Ivova; Kilminster, B.; MillanMejias, B.; Otiougova, P.; Robmann, P.; Snoek, H.; Taroni, S.; Tupputi, S.; Verzetti, M.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Li, S. W.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Dietz, C.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Suwonjandee, N.] Chulalongkorn Univ, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Karapinar, G.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Guelmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey. [Bahtiyar, H.; Barlas, E.; Cankocak, K.; Guenaydin, Y. O.; Vardarli, F. I.; Yucel, M.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Natl Sci Ctr, Kharkov Inst Phys & Technol, Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Kreczko, L.; Metson, S.; Newbold, D. M.; Nirunpong, K.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Basso, L.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Jackson, J.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Womersley, W. J.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Bainbridge, R.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.; Whyntie, T.] Univ London Imperial Coll Sci Technol & Med, London, England. [Chadwick, M.; Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; St John, J.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Bhattacharya, S.; Alimena, J.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Houtz, R.; Ko, W.; Kopecky, A.; Lander, R.; Mall, O.; Miceli, T.; Nelson, R.; Pellett, D.; Ricci-Tam, F.; Rutherford, B.; Searle, M.; Smith, J.; Squires, M.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Weber, M.; Andreev, V.; Cline, D.; Cousins, R.; Erhan, S.; Everaerts, P.; Farrell, C.; Felcini, M.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Rakness, G.; Schlein, P.; Takasugi, E.; Traczyk, P.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Liu, H.; Babb, J.; Clare, R.; Dinardo, M. E.; Ellison, J.; Gary, J. W.; Giordano, F.; Hanson, G.; Long, O. R.; Luthra, A.; Nguyen, H.; Paramesvaran, S.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sharma, V.; Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; Evans, D.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Macneill, I.; Mangano, B.; Padhi, S.; Palmer, C.; Petrucciani, G.; Pieri, M.; Sani, M.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bellan, R.; Campagnari, C.; D'Alfonso, M.; Danielson, T.; Flowers, K.; Geffert, P.; George, C.; Golf, F.; Incandela, J.; Justus, C.; Kalavase, P.; Kovalskyi, D.; Krutelyov, V.; Lowette, S.; Villalba, R. Magana; Mccoll, N.; Pavlunin, V.; Ribnik, J.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Di Marco, E.; Duarte, J.; Kcira, D.; Ma, Y.; Mott, A.; Newman, H. B.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Veverka, J.; Wilkinson, R.; Xie, S.; Yang, Y.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Liu, Y. F.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Eggert, N.; Gibbons, L. K.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Butler, P. H.; Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Gutsche, O.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Klima, B.; Kunori, S.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Wu, W.; Yang, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Chen, M.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Drozdetskiy, A.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Remington, R.; Rinkevicius, A.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Hewamanage, S.; Lebolo, L. M.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Gleyzer, S. V.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Callner, J.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Lacroix, F.; Moon, D. H.; O'Brien, C.; Silkworth, C.; Strom, D.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Griffiths, S.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Newsom, C. R.; Ogul, H.; Onel, Y.; Ozok, F.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Giurgiu, G.; Gritsan, A. V.; Hu, G.; Maksimovic, P.; Swartz, M.; Whitbeck, A.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Kenny, R. P., III; Murray, M.; Noonan, D.; Sanders, S.; Stringer, R.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Peterman, A.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Bauer, G.; Busza, W.; Butz, E.; Cali, I. A.; Chan, M.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Kim, Y.; Klute, M.; Lai, Y. S.; Levin, A.; Luckey, P. D.; Ma, T.; Nahn, S.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Sung, K.; Velicanu, D.; Wolf, R.; Wyslouch, B.; Yang, M.; Yilmaz, Y.; Yoon, A. S.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; De Benedetti, A.; Franzoni, G.; Gude, A.; Haupt, J.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Sasseville, M.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Cremaldi, L. M.; Kroeger, R.; Perera, L.; Rahmat, R.; Sanders, D. A.; Summers, D.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Eads, M.; Suarez, R. Gonzalez; Keller, J.; Kravchenko, I.; Lazo-Flores, J.; Malik, S.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Dolen, J.; Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Kumar, A.; Rappoccio, S.; Wan, Z.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Nash, D.; Orimoto, T.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Anastassov, A.; Hahn, K. A.; Kubik, A.; Lusito, L.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Berry, D.; Brinkerhoff, A.; Chan, K. M.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kolb, J.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Morse, D. M.; Pearson, T.; Planer, M.; Ruchti, R.; Slaunwhite, J.; Valls, N.; Wayne, M.; Wolf, M.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Bylsma, B.; Durkin, L. S.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Puigh, D.; Rodenburg, M.; Smith, G.; Vuosalo, C.; Williams, G.; Winer, B. L.; Wolfe, H.] Ohio State Univ, Columbus, OH 43210 USA. [Berry, E.; Elmer, P.; Halyo, V.; Hebda, P.; Hegeman, J.; Hunt, A.; Jindal, P.; Koay, S. A.; Pegna, D. 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Belyaev, Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279; Konecki, Marcin/0000-0001-9482-4841; Hernandez Calama, Jose Maria/0000-0001-6436-7547; Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680; Matorras, Francisco/0000-0003-4295-5668; Ragazzi, Stefano/0000-0001-8219-2074; Rovelli, Tiziano/0000-0002-9746-4842; TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; de Jesus Damiao, Dilson/0000-0002-3769-1680; Flix, Josep/0000-0003-2688-8047; Della Ricca, Giuseppe/0000-0003-2831-6982; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Paganoni, Marco/0000-0003-2461-275X; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Sznajder, Andre/0000-0001-6998-1108; Vilela Pereira, Antonio/0000-0003-3177-4626; Mundim, Luiz/0000-0001-9964-7805; Haj Ahmad, Wael/0000-0003-1491-0446; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Vieira de Castro Ferreira da Silva, Pedro Manuel/0000-0002-5725-041X; Androsov, Konstantin/0000-0003-2694-6542; Bean, Alice/0000-0001-5967-8674; Longo, Egidio/0000-0001-6238-6787; Di Matteo, Leonardo/0000-0001-6698-1735; Baarmand, Marc/0000-0002-9792-8619; Boccali, Tommaso/0000-0002-9930-9299; Menasce, Dario Livio/0000-0002-9918-1686; Bargassa, Pedrame/0000-0001-8612-3332; Attia Mahmoud, Mohammed/0000-0001-8692-5458; Bilki, Burak/0000-0001-9515-3306; Lloret Iglesias, Lara/0000-0002-0157-4765; Rolandi, Luigi (Gigi)/0000-0002-0635-274X; Sguazzoni, Giacomo/0000-0002-0791-3350; Casarsa, Massimo/0000-0002-1353-8964; Diemoz, Marcella/0000-0002-3810-8530; Tricomi, Alessia Rita/0000-0002-5071-5501; Ghezzi, Alessio/0000-0002-8184-7953; bianco, stefano/0000-0002-8300-4124; Demaria, Natale/0000-0003-0743-9465; Benaglia, Andrea Davide/0000-0003-1124-8450; Covarelli, Roberto/0000-0003-1216-5235; Ciulli, Vitaliano/0000-0003-1947-3396; Fiorendi, Sara/0000-0003-3273-9419; Martelli, Arabella/0000-0003-3530-2255; Gonzi, Sandro/0000-0003-4754-645X; Levchenko, Petr/0000-0003-4913-0538; Heath, Helen/0000-0001-6576-9740 FU BMWF (Austria); FWF (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MEYS (Bulgaria); CERN; CAS (China); MoST (China); NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); MoER (Estonia) [SF0690030s09]; ERDF (Estonia); Academy of Finland (Finland); MEC (Finland); HIP (Finland); CEA (France); CNRS/IN2P3 (France); BMBF (Germany); DFG (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NKTH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF (Republic of Korea); WCU (Republic of Korea); LAS (Lithuania); CINVESTAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); MSI (New Zealand); PAEC (Pakistan); MSHE (Poland); NSC (Poland); FCT (Portugal); JINR (Armenia); JINR (Belarus); JINR (Georgia); JINR (Ukraine); JINR (Uzbekistan); MON (Russia); RosAtom (Russia); RAS (Russia); RFBR (Russia); MSTD (Serbia); SEIDI (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); ThEPCenter (Thailand); IPST (Thailand); NSTDA (Thailand); TUBITAK (Turkey); TAEK (Turkey); NASU (Ukraine); STFC (United Kingdom); DOE (USA); NSF (USA); Marie-Curie programme (European Union); European Research Council (European Union); EPLANET (European Union); Leventis Foundation; A.P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of Czech Republic; Council of Science and Industrial Research, India; Compagnia di San Paolo (Torino); HOMING PLUS programme of Foundation for Polish Science; EU, Regional Development Fund; Thalis programme; Aristeia programme; EU-ESF; Greek NSRF FX We thank Gavin Salam for his valuable comments to this paper. We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centres and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWF and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ and FAPESP (Brazil); MEYS (Bulgaria); CERN; CAS, MoST and NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); MoER, SF0690030s09 and ERDF (Estonia); Academy of Finland, MEC and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG and HGF (Germany); GSRT (Greece); OTKA and NKTH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF and WCU (Republic of Korea); LAS (Lithuania); CINVESTAV, CONACYT, SEP and UASLP-FAI (Mexico); MSI (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Armenia, Belarus, Georgia, Ukraine, Uzbekistan); MON, RosAtom, RAS and RFBR (Russia); MSTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); ThEPCenter, IPST and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU (Ukraine); STFC (United Kingdom); DOE and NSF (USA).; Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A.P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of Czech Republic; the Council of Science and Industrial Research, India; the Compagnia di San Paolo (Torino); the HOMING PLUS programme of Foundation for Polish Science, cofinanced by EU, Regional Development Fund; and the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF. NR 43 TC 19 Z9 19 U1 3 U2 56 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD OCT 19 PY 2013 VL 73 IS 10 AR 2604 DI 10.1140/epjc/s10052-013-2604-6 PG 21 WC Physics, Particles & Fields SC Physics GA AC0JD UT WOS:000332179700001 ER PT J AU Subramanian, S Barry, AN Pieris, S Sayre, RT AF Subramanian, Sowmya Barry, Amanda N. Pieris, Shayani Sayre, Richard T. TI Comparative energetics and kinetics of autotrophic lipid and starch metabolism in chlorophytic microalgae: implications for biomass and biofuel production SO BIOTECHNOLOGY FOR BIOFUELS LA English DT Review DE Biofuel; Algae; Plant; Storage carbohydrate; Starch; Oil; Energetics; Photosynthesis; Biomass; Metabolism; Cultivation ID PHOTOSYNTHETIC QUANTUM YIELD; LIGHT-HARVESTING COMPLEX; CHLOROPLAST ATP SYNTHASE; PHOTOSYSTEM-II; CHLAMYDOMONAS-REINHARDTII; CRYSTAL-STRUCTURE; CHLORELLA-PROTOTHECOIDES; BIODIESEL PRODUCTION; ENERGY-TRANSFER; CARBON-DIOXIDE AB Due to the growing need to provide alternatives to fossil fuels as efficiently, economically, and sustainably as possible there has been growing interest in improved biofuel production systems. Biofuels produced from microalgae are a particularly attractive option since microalgae have production potentials that exceed the best terrestrial crops by 2 to 10-fold. In addition, autotrophically grown microalgae can capture CO2 from point sources reducing direct atmospheric greenhouse gas emissions. The enhanced biomass production potential of algae is attributed in part to the fact that every cell is photosynthetic. Regardless, overall biological energy capture, conversion, and storage in microalgae are inefficient with less than 8% conversion of solar into chemical energy achieved. In this review, we examine the thermodynamic and kinetic constraints associated with the autotrophic conversion of inorganic carbon into storage carbohydrate and oil, the dominant energy storage products in Chlorophytic microalgae. We discuss how thermodynamic restrictions including the loss of fixed carbon during acetyl CoA synthesis reduce the efficiency of carbon accumulation in lipids. In addition, kinetic limitations, such as the coupling of proton to electron transfer during plastoquinone reduction and oxidation and the slow rates of CO2 fixation by Rubisco reduce photosynthetic efficiency. In some cases, these kinetic limitations have been overcome by massive increases in the numbers of effective catalytic sites, e. g. the high Rubisco levels (mM) in chloroplasts. But in other cases, including the slow rate of plastoquinol oxidation, there has been no compensatory increase in the abundance of catalytically limiting protein complexes. Significantly, we show that the energetic requirements for producing oil and starch relative to the recoverable energy stored in these molecules are very similar on a per carbon basis. Presently, the overall rates of starch and lipid synthesis in microalgae are very poorly characterized. Increased understanding of the kinetic constraints of lipid and starch synthesis, accumulation and turnover would facilitate the design of improved biomass production systems. C1 [Subramanian, Sowmya; Sayre, Richard T.] New Mexico Consortium, Biosci Div, Los Alamos, NM 87544 USA. [Barry, Amanda N.; Sayre, Richard T.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Pieris, Shayani] Missouri Baptist Univ, Div Nat Sci, St Louis, MO 63141 USA. RP Pieris, S (reprint author), Missouri Baptist Univ, Div Nat Sci, 1 Coll Pk Dr, St Louis, MO 63141 USA. EM shayanipieris@gmail.com; rsayre@newmexicoconsortium.org OI Sayre, Richard/0000-0002-3153-7084; Barry, Amanda/0000-0002-7992-0322 FU US-DOE Center for Advanced Biofuels [DE SC0001295]; Los Alamos Laboratory LDRD program; US Air Force Office of Scientific Research [FA9550-08-1-0451]; US DOE National Alliance for Advanced Biofuels and Bioproducts [DE-EE0003046]; US-DOE-EFRC, Center for Advanced Biofuels [DE-SC0001295] FX Sowmya Subramanian was supported by US-DOE Center for Advanced Biofuels contract, DE SC0001295.; Amanda N. Barry was supported by the Los Alamos Laboratory LDRD program.; Shayani Pieris was supported by the US Air Force Office of Scientific Research, contract FA9550-08-1-0451.; Richard Sayre was supported by US DOE National Alliance for Advanced Biofuels and Bioproducts, contract, DE-EE0003046, and by the US-DOE-EFRC, Center for Advanced Biofuels, contract, DE-SC0001295. NR 102 TC 20 Z9 20 U1 6 U2 108 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1754-6834 J9 BIOTECHNOL BIOFUELS JI Biotechnol. Biofuels PD OCT 19 PY 2013 VL 6 AR 150 DI 10.1186/1754-6834-6-150 PG 12 WC Biotechnology & Applied Microbiology; Energy & Fuels SC Biotechnology & Applied Microbiology; Energy & Fuels GA 247VX UT WOS:000326652100001 PM 24139286 ER PT J AU Majorek, KA Kuhn, ML Chruszcz, M Anderson, WF Minor, W AF Majorek, Karolina A. Kuhn, Misty L. Chruszcz, Maksymilian Anderson, Wayne F. Minor, Wladek TI Structural, Functional, and Inhibition Studies of a Gcn5-related N-Acetyltransferase (GNAT) Superfamily Protein PA4794 A NEW C-TERMINAL LYSINE PROTEIN ACETYLTRANSFERASE FROM PSEUDOMONAS AERUGINOSA SO JOURNAL OF BIOLOGICAL CHEMISTRY LA English DT Article DE Antibiotics; Crystal Structure; Enzyme inhibitors; High Throughput Screening (HTS); Pseudomonas; GNAT; Gcn5-related N-Acetyltransferase; Acetyltransferase; Cephalosporin; Lysine Acetylation ID X-RAY-DIFFRACTION; SALMONELLA-TYPHIMURIUM; ACETYLATION; MODEL; COOT AB Background: Gcn5-related N-acetyltransferases (GNATs) are involved in small molecule and protein acetylation in all organisms. Results: Crystallographic and biochemical characterization of PA4794 is shown, including identification of substrates and inhibitors. Conclusion: PA4794 is a new bacterial C-terminal lysine protein acetyltransferase inhibited by cephalosporins. Significance: PA4794 is the first identified acetyltransferase specific for C-terminal lysine; identified interactions with cephalosporins may be of clinical relevance. The Gcn5-related N-acetyltransferase (GNAT) superfamily is a large group of evolutionarily related acetyltransferases, with multiple paralogs in organisms from all kingdoms of life. The functionally characterized GNATs have been shown to catalyze the transfer of an acetyl group from acetyl-coenzyme A (Ac-CoA) to the amine of a wide range of substrates, including small molecules and proteins. GNATs are prevalent and implicated in a myriad of aspects of eukaryotic and prokaryotic physiology, but functions of many GNATs remain unknown. In this work, we used a multi-pronged approach of x-ray crystallography and biochemical characterization to elucidate the sequence-structure-function relationship of the GNAT superfamily member PA4794 from Pseudomonas aeruginosa. We determined that PA4794 acetylates the NE amine of a C-terminal lysine residue of a peptide, suggesting it is a protein acetyltransferase specific for a C-terminal lysine of a substrate protein or proteins. Furthermore, we identified a number of molecules, including cephalosporin antibiotics, which are inhibitors of PA4794 and bind in its substrate-binding site. Often, these molecules mimic the conformation of the acetylated peptide product. We have determined structures of PA4794 in the apo-form, in complexes with Ac-CoA, CoA, several antibiotics and other small molecules, and a ternary complex with the products of the reaction: CoA and acetylated peptide. Also, we analyzed PA4794 mutants to identify residues important for substrate binding and catalysis. C1 [Majorek, Karolina A.; Chruszcz, Maksymilian; Minor, Wladek] Univ Virginia, Dept Mol Physiol & Biol Phys, Charlottesville, VA 22908 USA. [Majorek, Karolina A.] Adam Mickiewicz Univ, Bioinformat Lab, Inst Mol Biol & Biotechnol, Fac Biol, PL-61614 Poznan, Poland. [Kuhn, Misty L.; Anderson, Wayne F.] Northwestern Univ, Dept Mol Pharmacol & Biol Chem, Feinberg Sch Med, Chicago, IL 60611 USA. [Chruszcz, Maksymilian] Univ S Carolina, Dept Chem & Biochem, Columbia, SC 29208 USA. [Majorek, Karolina A.; Chruszcz, Maksymilian; Anderson, Wayne F.; Minor, Wladek] Argonne Natl Lab, Midwest Ctr Struct Genom, Argonne, IL 60439 USA. RP Minor, W (reprint author), Univ Virginia, Dept Mol Physiol & Biol Phys, 1340 Jefferson Pk Ave, Charlottesville, VA 22908 USA. EM wladek@iwonka.med.virginia.edu RI Minor, Wladek/F-3096-2014; OI Chruszcz, Maksymilian/0000-0001-7521-5485; Minor, Wladek/0000-0001-7075-7090 FU United States DOE Office of Biological and Environmental Research [DE-AC02-06CH11357]; Michigan Technology Tri-Corridor Grant [085P1000817] FX We thank Dr. Igor Shumilin and Przemyslaw Porebski for valuable discussions and Dr. Matthew D. Zimmerman for critically reading the manuscript. Additionally, we thank Drs. Sergii Pshenychnyi and Izolda Popova at the Recombinant Protein Production Core at Northwestern University for expression and purification services. Some results shown in this report are derived from work performed at the Structural Biology Center Sector 19 and LS-CAT Sector 21 at the Advanced Photon Source. The Advanced Photon Source, an Office of Science User Facility, is operated for the United States Dept. of Energy (DOE) Office of Science by Argonne National Laboratory. Argonne is operated by University of Chicago Argonne, LLC, for the United States DOE Office of Biological and Environmental Research under contract DE-AC02-06CH11357. Use of LS-CAT Sector 21 was also supported by the Michigan Economic Development Corporation and the Michigan Technology Tri-Corridor Grant 085P1000817 NR 35 TC 14 Z9 14 U1 2 U2 14 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 0021-9258 EI 1083-351X J9 J BIOL CHEM JI J. Biol. Chem. PD OCT 18 PY 2013 VL 288 IS 42 BP 30223 EP 30235 DI 10.1074/jbc.M113.501353 PG 13 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA 291YF UT WOS:000329868100021 PM 24003232 ER PT J AU Varjas, D Zaletel, MP Moore, JE AF Varjas, Daniel Zaletel, Michael P. Moore, Joel E. TI Chiral Luttinger liquids and a generalized Luttinger theorem in fractional quantum Hall edges via finite-entanglement scaling SO PHYSICAL REVIEW B LA English DT Article ID LANDAU-LEVEL; STATES; EXCITATIONS; SYSTEMS; TRANSPORT AB We use bosonic field theories and the infinite system density matrix renormalization group method to study infinite strips of fractional quantum Hall states starting from microscopic Hamiltonians. Finite-entanglement scaling allows us to accurately measure chiral central charge, edge-mode exponents, and momenta without finite-size errors. We analyze states in the first and second levels of the standard hierarchy and compare our results to predictions of the chiral Luttinger liquid theory. The results confirm the universality of scaling exponents in chiral edges and demonstrate that renormalization is subject to universal relations in the nonchiral case. We prove a generalized Luttinger theorem involving all singularities in the momentum-resolved density, which naturally arises when mapping Landau levels on a cylinder to a fermion chain and deepens our understanding of non-Fermi liquids in one dimension. C1 [Varjas, Daniel; Zaletel, Michael P.; Moore, Joel E.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Moore, Joel E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Varjas, D (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. RI Moore, Joel/O-4959-2016 OI Moore, Joel/0000-0002-4294-5761 FU NSF GRFP [DGE 1106400]; NSF [DMR-1206515] FX We thank S. Parameswaran, R. Mong, F. D. M. Haldane, and J. Jain for useful discussions. M.P.Z. acknowledges support from NSF GRFP Grant No. DGE 1106400. D. V. and J. E. M. acknowledge support from NSF Grant No. DMR-1206515. NR 54 TC 4 Z9 4 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD OCT 18 PY 2013 VL 88 IS 15 AR 155314 DI 10.1103/PhysRevB.88.155314 PG 8 WC Physics, Condensed Matter SC Physics GA 240HB UT WOS:000326084800003 ER PT J AU Hooper, D AF Hooper, Dan TI Is the cosmic microwave background telling us that dark matter is weaker than weakly interacting? SO PHYSICAL REVIEW D LA English DT Article ID BARYON ACOUSTIC-OSCILLATIONS; DIGITAL SKY SURVEY; COSMOLOGICAL IMPLICATIONS; SUPERSYMMETRY BREAKING; HUBBLE CONSTANT; ABUNDANCES; GRAVITINO; DILATION; DISTANCE; POLONYI AB If moduli, or other long-lived heavy states, decay in the early universe in part into light and feebly interacting particles (such as axions), these decay products could account for the additional energy density in radiation that is suggested by recent measurements of the cosmic microwave background. These moduli decays will also, however, alter the thermal history of the early universe, potentially reducing the thermal relic abundance of dark matter. If this is the case, then dark matter particles must annihilate with an even lower cross section than required in the standard thermal scenario (>> 3 x 10(-26) cm(3)/s) if they are to make up the observed density of dark matter. This possibility has significant implications for direct and indirect searches for dark matter. C1 [Hooper, Dan] Fermilab Natl Accelerator Lab, Ctr Particle Astrophys, Batavia, IL 60510 USA. [Hooper, Dan] Univ Chicago, Dept Astron & Astrophys, Chicago, IL 60637 USA. RP Hooper, D (reprint author), Fermilab Natl Accelerator Lab, Ctr Particle Astrophys, POB 500, Batavia, IL 60510 USA. FU U.S. Department of Energy FX The author would like to thank Scott Watson, Lisa Randall, and Graciela Gelmini for valuable discussions, and the Kavli Institute for Theoretical Physics for their hospitality. This work has been supported by the U.S. Department of Energy. NR 64 TC 8 Z9 8 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD OCT 18 PY 2013 VL 88 IS 8 AR 083519 DI 10.1103/PhysRevD.88.083519 PG 5 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 240NQ UT WOS:000326104100005 ER PT J AU Hooper, D Cholis, I Linden, T Siegal-Gaskins, JM Slatyer, TR AF Hooper, Dan Cholis, Ilias Linden, Tim Siegal-Gaskins, Jennifer M. Slatyer, Tracy R. TI Millisecond pulsars cannot account for the inner Galaxy's GeV excess SO PHYSICAL REVIEW D LA English DT Article ID LARGE-AREA TELESCOPE; X-RAY BINARIES; GALACTIC-CENTER; SOURCE CATALOG; DARK-MATTER; POPULATION; COLLAPSE; SUPERNOVAE; RADIO; SKY AB Using data from the Fermi Gamma-Ray Space Telescope, a spatially extended component of gamma rays has been identified from the direction of the Galactic center, peaking at energies of similar to 2-3 GeV. More recently, it has been shown that this signal is not confined to the innermost hundreds of parsecs of the Galaxy, but instead extends to at least similar to 3 kpc from the Galactic center. While the spectrum, intensity, and angular distribution of this signal is in good agreement with predictions from annihilating dark matter, it has also been suggested that a population of unresolved millisecond pulsars could be responsible for this excess GeV emission from the inner Galaxy. In this paper, we consider this later possibility in detail. Comparing the observed spectral shape of the inner Galaxy's GeV excess to the spectrum measured from 37 millisecond pulsars by Fermi, we find that these sources exhibit a spectral shape that is much too soft at sub-GeV energies to accommodate this signal. We also construct population models to describe the spatial distribution and luminosity function of the Milky Way's millisecond pulsars. After taking into account constraints from the observed distribution of Fermi sources ( including both sources known to be millisecond pulsars, and unidentified sources which could be pulsars), we find that millisecond pulsars can account for no more than similar to 10% of the inner Galaxy's GeV excess. Each of these arguments strongly disfavor millisecond pulsars as the source of this signal. C1 [Hooper, Dan; Cholis, Ilias] Fermilab Natl Accelerator Lab, Ctr Particle Astrophys, Batavia, IL 60510 USA. [Hooper, Dan] Univ Chicago, Dept Astron & Astrophys, Chicago, IL 60637 USA. [Linden, Tim] Univ Calif Santa Cruz, Dept Phys, Santa Cruz, CA 95064 USA. [Siegal-Gaskins, Jennifer M.] CALTECH, Pasadena, CA 91125 USA. [Slatyer, Tracy R.] Inst Adv Study, Sch Nat Sci, Princeton, NJ 08540 USA. RP Hooper, D (reprint author), Fermilab Natl Accelerator Lab, Ctr Particle Astrophys, POB 500, Batavia, IL 60510 USA. FU U.S. Department of Energy; National Science Foundation [PHY-0907744, AST-0807444]; NASA through Einstein Postdoctoral Fellowship [PF1-120089]; Chandra X-ray Center, which is operated by the Smithsonian Astrophysical Observatory for NASA [NAS8-03060] FX We would like to thank Manoj Kaplinghat, Kev Abazajian, and Albert Stebbins for helpful discussions. This work has been supported by the U.S. Department of Energy. T.R.S. is supported by the National Science Foundation under Grants No. PHY-0907744 and No. AST-0807444. J.M.S.G. acknowledges support from NASA through Einstein Postdoctoral Fellowship Grant No. PF1-120089 awarded by the Chandra X-ray Center, which is operated by the Smithsonian Astrophysical Observatory for NASA under Contract No. NAS8-03060. NR 36 TC 92 Z9 92 U1 1 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD OCT 18 PY 2013 VL 88 IS 8 AR 083009 DI 10.1103/PhysRevD.88.083009 PG 12 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 240NQ UT WOS:000326104100002 ER PT J AU Lin, SZ Batista, CD AF Lin, Shi-Zeng Batista, Cristian D. TI Orbital Magnetism Induced by Heat Currents in Mott Insulators SO PHYSICAL REVIEW LETTERS LA English DT Article ID SPIN; PHASE; FERROMAGNET; ENERGY; STATES AB We derive the effective heat current density operator for the strong-coupling regime of Mott insulators. Similarly to the case of the electric current density, the leading contribution to this effective operator is proportional to the local scalar spin chirality (chi) over cap (jkl) = S-l.(S-j x S-k). This common form of the effective heat and electric current density operators leads to a novel cross response in Mott insulators. A heat current induces a distribution of orbital magnetic moments in systems containing loops of an odd number of hopping terms. The relative orientation of the orbital moments depends on the particular lattice of magnetic ions. This subtle effect arises from the symmetries that the heat and electric currents have in common. C1 [Lin, Shi-Zeng; Batista, Cristian D.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Lin, SZ (reprint author), Los Alamos Natl Lab, Div Theoret, T4, Los Alamos, NM 87545 USA. RI Lin, Shi-Zeng/B-2906-2008; Batista, Cristian/J-8008-2016 OI Lin, Shi-Zeng/0000-0002-4368-5244; FU NNSA of the U.S. DOE at LANL [DE-AC52-06NA25396]; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering FX This work was carried out under the auspices of the NNSA of the U.S. DOE at LANL under Award No. DE-AC52-06NA25396, and was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. NR 25 TC 2 Z9 2 U1 1 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 18 PY 2013 VL 111 IS 16 AR 166602 DI 10.1103/PhysRevLett.111.166602 PG 5 WC Physics, Multidisciplinary SC Physics GA 241EA UT WOS:000326148000014 PM 24182288 ER PT J AU Unger, SD Rhodes, OE Sutton, TM Williams, RN AF Unger, Shem D. Rhodes, Olin E., Jr. Sutton, Trent M. Williams, Rod N. TI Population Genetics of the Eastern Hellbender (Cryptobranchus alleganiensis alleganiensis) across Multiple Spatial Scales SO PLOS ONE LA English DT Article ID MICROSATELLITE DNA VARIATION; LANDSCAPE GENETICS; SALVELINUS-FONTINALIS; CONSERVATION GENETICS; AMPHIBIAN DECLINES; ATLANTIC SALMON; STREAM NETWORKS; F-STATISTICS; BROOK CHARR; DIVERSITY AB Conservation genetics is a powerful tool to assess the population structure of species and provides a framework for informing management of freshwater ecosystems. As lotic habitats become fragmented, the need to assess gene flow for species of conservation management becomes a priority. The eastern hellbender (Cryptobranchus alleganiensis alleganiensis) is a large, fully aquatic paedamorphic salamander. Many populations are experiencing declines throughout their geographic range, yet the genetic ramifications of these declines are currently unknown. To this end, we examined levels of genetic variation and genetic structure at both range-wide and drainage (hierarchical) scales. We collected 1,203 individuals from 77 rivers throughout nine states from June 2007 to August 2011. Levels of genetic diversity were relatively high among all sampling locations. We detected significant genetic structure across populations (Fst values ranged from 0.001 between rivers within a single watershed to 0.218 between states). We identified two genetically differentiated groups at the range-wide scale: 1) the Ohio River drainage and 2) the Tennessee River drainage. An analysis of molecular variance (AMOVA) based on landscape-scale sampling of basins within the Tennessee River drainage revealed the majority of genetic variation (similar to 94-98%) occurs within rivers. Eastern hellbenders show a strong pattern of isolation by stream distance (IBSD) at the drainage level. Understanding levels of genetic variation and differentiation at multiple spatial and biological scales will enable natural resource managers to make more informed decisions and plan effective conservation strategies for cryptic, lotic species. C1 [Unger, Shem D.; Rhodes, Olin E., Jr.] Univ Georgia, Savannah River Ecol Lab, Aiken, SC USA. [Sutton, Trent M.] Univ Alaska Fairbanks, Sch Fisheries & Ocean Sci, Fairbanks, AK USA. [Williams, Rod N.] Purdue Univ, Dept Forestry & Nat Resources, W Lafayette, IN 47907 USA. RP Unger, SD (reprint author), Univ Georgia, Savannah River Ecol Lab, Aiken, SC USA. EM cryptobranchus11@gmail.com FU Indiana Department of Natural Resources [E2-07-WD0007]; Department of Forestry and Natural Resources at Purdue University; Cryptobranchid Interest Group Ron Goellner Fund FX Funding was provided by the Indiana Department of Natural Resources (E2-07-WD0007; http://www.in.gov/dnr/), Department of Forestry and Natural Resources at Purdue University (https://ag.purdue.edu/fnr/Pages/default.aspx), and Cryptobranchid Interest Group Ron Goellner Fund (2010; http://www.caudata.org/cig/). The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 82 TC 6 Z9 6 U1 4 U2 46 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD OCT 18 PY 2013 VL 8 IS 10 AR e74180 DI 10.1371/journal.pone.0074180 PG 14 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 239MM UT WOS:000326029300002 PM 24204565 ER PT J AU Wright, JB Liu, S Wang, GT Li, QM Benz, A Koleske, DD Lu, P Xu, HW Lester, L Luk, TS Brener, I Subramania, G AF Wright, Jeremy B. Liu, Sheng Wang, George T. Li, Qiming Benz, Alexander Koleske, Daniel D. Lu, Ping Xu, Huiwen Lester, Luke Luk, Ting S. Brener, Igal Subramania, Ganapathi TI Multi-Colour Nanowire Photonic Crystal Laser Pixels SO SCIENTIFIC REPORTS LA English DT Article ID STIMULATED-EMISSION; NANOCOLUMN ARRAYS; MODE LASER; CONFINEMENT AB Emerging applications such as solid-state lighting and display technologies require micro-scale vertically emitting lasers with controllable distinct lasing wavelengths and broad wavelength tunability arranged in desired geometrical patterns to form "super-pixels". Conventional edge-emitting lasers and current surface-emitting lasers that require abrupt changes in semiconductor bandgaps or cavity length are not a viable solution. Here, we successfully address these challenges by introducing a new paradigm that extends the laser tuning range additively by employing multiple monolithically grown gain sections each with a different emission centre wavelength. We demonstrate this using broad gain-bandwidth III-nitride multiple quantum well (MQW) heterostructures and a novel top-down nanowire photonic crystal nanofabrication. We obtain single-mode lasing in the blue-violet spectral region with a remarkable 60 nm of tuning (or 16% of the nominal centre wavelength) that is determined purely by the photonic crystal geometry. This approach can be extended to cover the entire visible spectrum. C1 [Wright, Jeremy B.; Liu, Sheng; Wang, George T.; Li, Qiming; Benz, Alexander; Koleske, Daniel D.; Lu, Ping; Luk, Ting S.; Brener, Igal; Subramania, Ganapathi] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Wright, Jeremy B.; Xu, Huiwen; Lester, Luke] Univ New Mexico, Ctr High Technol Mat, Albuquerque, NM 87106 USA. [Luk, Ting S.; Brener, Igal] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87123 USA. [Lester, Luke; Subramania, Ganapathi] Univ New Mexico, Dept Elect & Comp Engn, Albuquerque, NM 87131 USA. RP Subramania, G (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM gssubra@sandia.gov RI Wright, Jeremy/G-7149-2011; Liu, Sheng/P-6029-2014 OI Wright, Jeremy/0000-0001-6861-930X; Liu, Sheng/0000-0003-0967-4514 FU Sandia's Solid-State-Lighting Science Energy Frontier Research Center; U.S. Department of Energy, Office of Science, and Office of Basic Energy Sciences; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors would like to thank Karen Cross and Jason Dominguez for their help with the fabrication of the 2DPC samples. The authors would like to thank Jeff Tsao for his useful discussions and help with the manuscript. This work was supported by Sandia's Solid-State-Lighting Science Energy Frontier Research Center, funded by the U.S. Department of Energy, Office of Science, and Office of Basic Energy Sciences. This work was performed, in part, at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the U. S. Department of Energy (DOE) Office of Science. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 21 TC 23 Z9 23 U1 2 U2 38 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD OCT 18 PY 2013 VL 3 AR 2982 DI 10.1038/srep02982 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 237IZ UT WOS:000325864300003 PM 24135975 ER PT J AU Chen, MC Huang, JR Mahanthappa, KT Wijangco, AM AF Chen, Mu-Chun Huang, Jinrui Mahanthappa, K. T. Wijangco, Alexander M. TI Large theta(13) in a SUSY SU(5) x T ' model SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Beyond Standard Model; Neutrino Physics; Discrete and Finite Symmetries; GUT ID DISCRETE FLAVOR SYMMETRIES; A(4) FAMILY SYMMETRY; PARTICLE PHYSICS; NEUTRINO MASSES; FERMION MASSES; QUARK MASSES; CP VIOLATION; CKM; PREDICTIONS; ANOMALIES AB In the model based on SUSY SU(5) combined with the T' family symmetry, it is shown [1, 2] that fermion mass hierarchy and mixing angles can be naturally generated in both lepton and quark sectors compatible with various experimental measurements. But the predicted value for the non-zero lepton mixing angle of theta(13) similar or equal to theta(c)/3 root 2 contradicts the recent experimental results from Daya Bay and RENO. We propose to introduce one more singlet flavon field in the neutrino sector, and with its additional contribution, we are able to generate the large mixing angle theta(13) similar to 8 degrees - 10 degrees. The analytical expressions of the mixing angles and neutrino masses with the additional flavon field are derived. Our numerical results show that a large region in the model parameter space is allowed for the normal hierarchy case, while a much smaller region is allowed for the inverted hierarchy case. In addition, the predicted value of the solar mixing angle is not affected by the additional singlet contribution. On the other hand, there exists a correlation between 013 value and theta(23) - pi/4, as a result of the additional singlet contribution. We also make predictions for various other variables that can be potentially tested in the future neutrino experiments such as the Dirac CP phase, which is predicted to be in the range of delta similar to (195 degrees - 200 degrees), and the neutrinoless double beta decay matrix element, < m(beta beta)>. One numerical example with the minimal chi(2) fit is presented, and the model predictions are consistent with all experimental results. C1 [Chen, Mu-Chun; Wijangco, Alexander M.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. [Huang, Jinrui] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Mahanthappa, K. T.] Univ Colorado, Dept Phys, Boulder, CO 80309 USA. RP Chen, MC (reprint author), Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. EM muchunc@uci.edu; jinruih@lanl.gov; ktm@pizero.colorado.edu; awijangc@uci.edu RI Huang, Jinrui/O-2439-2013 FU National Science Foundation [PHY-0970173]; Department of Energy [DE-FG02-04ER41290]; DOE Office of Science; LANL LDRD program FX We thank Michael Ratz for useful comments. The work of M-CC and A.M.W. was supported, in part, by the National Science Foundation under Grant No. PHY-0970173. The work of KTM was supported, in part, by the Department of Energy under Grant No. DE-FG02-04ER41290. JH is supported by the DOE Office of Science and the LANL LDRD program. A.M.W. would also like to acknowledge the hospitality of the TASI Summer School, where part of this work was completed. NR 65 TC 7 Z9 7 U1 0 U2 1 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD OCT 18 PY 2013 IS 10 AR UNSP 112 DI 10.1007/JHEP10(2013)112 PG 19 WC Physics, Particles & Fields SC Physics GA 236SF UT WOS:000325818800002 ER PT J AU Fallis, J Parikh, A Bertone, PF Bishop, S Buchmann, L Chen, AA Christian, G Clark, JA D'Auria, JM Davids, B Deibel, CM Fulton, BR Greife, U Guo, B Hager, U Herlitzius, C Hutcheon, DA Jose, J Laird, AM Li, ET Li, ZH Lian, G Liu, WP Martin, L Nelson, K Ottewell, D Parker, PD Reeve, S Rojas, A Ruiz, C Setoodehnia, K Sjue, S Vockenhuber, C Wang, YB Wrede, C AF Fallis, J. Parikh, A. Bertone, P. F. Bishop, S. Buchmann, L. Chen, A. A. Christian, G. Clark, J. A. D'Auria, J. M. Davids, B. Deibel, C. M. Fulton, B. R. Greife, U. Guo, B. Hager, U. Herlitzius, C. Hutcheon, D. A. Jose, J. Laird, A. M. Li, E. T. Li, Z. H. Lian, G. Liu, W. P. Martin, L. Nelson, K. Ottewell, D. Parker, P. D. Reeve, S. Rojas, A. Ruiz, C. Setoodehnia, K. Sjue, S. Vockenhuber, C. Wang, Y. B. Wrede, C. TI Constraining nova observables: Direct measurements of resonance strengths in 33S(p,gamma)34Cl SO PHYSICAL REVIEW C LA English DT Article ID CLASSICAL NOVAE; PRESOLAR GRAINS; DRAGON FACILITY; REACTION-RATES; NUCLEOSYNTHESIS; CHEMISTRY; NUCLEI; ISAC; GAS AB The S-33(p,gamma)Cl-34 reaction is important for constraining predictions of certain isotopic abundances in oxygenneon novae. Models currently predict as much as 150 times the solar abundance of S-33 in oxygen-neon nova ejecta. This overproduction factor may vary by orders of magnitude due to uncertainties in the S-33(p,gamma)Cl-34 reaction rate at nova peak temperatures. Depending on this rate, S-33 could potentially be used as a diagnostic tool for classifying certain types of presolar grains. Better knowledge of the S-33(p,gamma)(34) rate would also aid in interpreting nova observations over the S-Ca mass region and contribute to the firm establishment of the maximum endpoint of nova nucleosynthesis. Additionally, the total S elemental abundance which is affected by this reaction has been proposed as a thermometer to study the peak temperatures of novae. Previously, the S-33(p,gamma)(34) reaction rate had only been studied directly down to resonance energies of 432 keV. However, for nova peak temperatures of 0.2-0.4 GK there are seven known states in Cl-34 both below the 432-keV resonance and within the Gamow window that could play a dominant role. Direct measurements of the resonance strengths of these states were performed using the DRAGON (Detector of Recoils And Gammas of Nuclear reactions) recoil separator at TRIUMF. Additionally two new states within this energy region are reported. Several hydrodynamic simulations have been performed, using all available experimental information for the S-33(p,gamma)(34) rate, to explore the impact of the remaining uncertainty in this rate on nucleosynthesis in nova explosions. These calculations give a range of approximate to 20-150 for the expected S-33 overproduction factor, and a range of approximate to 100-450 for the S-32/S-33 ratio expected in ONe novae. C1 [Fallis, J.; Buchmann, L.; Christian, G.; Davids, B.; Hager, U.; Hutcheon, D. A.; Martin, L.; Nelson, K.; Ottewell, D.; Reeve, S.; Rojas, A.; Ruiz, C.; Sjue, S.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Parikh, A.; Jose, J.] Univ Politecn Cataluna, EUETIB, Dept Fis & Engn Nucl, E-08036 Barcelona, Spain. [Parikh, A.; Jose, J.] Inst Estudis Espacials Catalunya, E-08034 Barcelona, Spain. [Parikh, A.; Herlitzius, C.] Tech Univ Munich, Phys Dept E12, D-85748 Garching, Germany. [Bertone, P. F.; Clark, J. A.; Deibel, C. M.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Chen, A. A.; Nelson, K.; Setoodehnia, K.] McMaster Univ, Hamilton, ON, Canada. [D'Auria, J. M.; Davids, B.; Reeve, S.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Deibel, C. M.] Michigan State Univ, Joint Inst Nucl Astrophys, E Lansing, MI 48824 USA. [Deibel, C. M.] Louisiana State Univ, Dept Phys & Astron, Baton Rouge, LA 70803 USA. [Fulton, B. R.; Laird, A. M.] Univ York, Dept Phys, York YO10 5DD, N Yorkshire, England. [Greife, U.; Hager, U.] Colorado Sch Mines, Golden, CO 80401 USA. [Guo, B.; Li, E. T.; Li, Z. H.; Lian, G.; Liu, W. P.; Wang, Y. B.] China Inst Atom Energy, Beijing 102413, Peoples R China. [Parker, P. D.] Yale Univ, Wright Nucl Struct Lab, New Haven, CT 06520 USA. [Vockenhuber, C.] ETH, Zurich, Switzerland. [Wrede, C.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Wrede, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Wrede, C.] Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA. RP Fallis, J (reprint author), TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. EM jfallis@trumf.ca RI Hager, Ulrike/O-1738-2016 FU Natural Sciences and Engineering Research Council of Canada; Spanish MICINN [AYA2010-15685, EUI2009-04167]; Government of Catalonia [2009SGR-1002]; E.U. FEDER funds; ESF EUROCORES Program EuroGENESIS; DFG; Department of Energy, Office of Nuclear Physics [DE-AC02-06CH11357]; National Science Foundation; Science and Technology Funding Council; National Natural Science Foundation of China [11021504]; 973 Program of China [2013CB834406] FX We thank the beam delivery and ISAC operations groups at TRIUMF and also gratefully acknowledge the invaluable assistance in beam production from K. Jayamanna. The authors gratefully acknowledge funding from the Natural Sciences and Engineering Research Council of Canada. A.P. and J.J. were partially supported by the Spanish MICINN Grants No. AYA2010-15685 and No. EUI2009-04167, the Government of Catalonia Grant No. 2009SGR-1002, the E.U. FEDER funds, and the ESF EUROCORES Program EuroGENESIS. A.P. was also supported by the DFG cluster of excellence "Origin and Structure of the Universe." Authors from the USA thank both the Department of Energy, Office of Nuclear Physics (Contract No. DE-AC02-06CH11357), and the National Science Foundation for their support. Authors from the UK aknowledge the support of the Science and Technology Funding Council. Collaborators from CIAE thank the National Natural Science Foundation of China (Grant No. 11021504) and the 973 Program of China (Grant No. 2013CB834406). NR 35 TC 9 Z9 9 U1 0 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD OCT 18 PY 2013 VL 88 IS 4 AR 045801 DI 10.1103/PhysRevC.88.045801 PG 11 WC Physics, Nuclear SC Physics GA 240KX UT WOS:000326095900003 ER PT J AU Grady, NK Perkins, BG Hwang, HY Brandt, NC Torchinsky, D Singh, R Yan, L Trugman, D Trugman, SA Jia, QX Taylor, AJ Nelson, KA Chen, HT AF Grady, Nathaniel K. Perkins, Bradford G., Jr. Hwang, Harold Y. Brandt, Nathaniel C. Torchinsky, Darius Singh, Ranjan Yan, Li Trugman, Daniel Trugman, Stuart A. Jia, Q. X. Taylor, Antoinette J. Nelson, Keith A. Chen, Hou-Tong TI Nonlinear high-temperature superconducting terahertz metamaterials SO NEW JOURNAL OF PHYSICS LA English DT Article ID MICROSTRIP RESONATOR; NEGATIVE INDEX; PAIR-BREAKING; REFRACTION; TRANSITION; FILMS; YBA2CU3O7-DELTA; INTERMODULATION; CURRENTS; FIELDS AB We report the observation of a nonlinear terahertz response of splitring resonator arrays made of high-temperature superconducting films. Intensity-dependent transmission measurements indicate that the resonance strength decreases dramatically (i.e. transient bleaching) and the resonance frequency shifts as the intensity is increased. Pump-probe measurements confirm this behaviour and reveal dynamics on the few-picosecond timescale. C1 [Grady, Nathaniel K.; Singh, Ranjan; Yan, Li; Trugman, Daniel; Trugman, Stuart A.; Jia, Q. X.; Taylor, Antoinette J.; Chen, Hou-Tong] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. [Perkins, Bradford G., Jr.; Hwang, Harold Y.; Brandt, Nathaniel C.; Torchinsky, Darius; Nelson, Keith A.] MIT, Dept Chem, Cambridge, MA 02139 USA. RP Chen, HT (reprint author), Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. EM chenht@lanl.gov RI Grady, Nathaniel/A-4896-2011; Chen, Hou-Tong/C-6860-2009; Singh, Ranjan/B-4091-2010; Jia, Q. X./C-5194-2008; OI Grady, Nathaniel/0000-0002-0885-3337; Chen, Hou-Tong/0000-0003-2014-7571; Singh, Ranjan/0000-0001-8068-7428; Trugman, Stuart/0000-0002-6688-7228 FU Los Alamos National Laboratory's Laboratory Directed Research and Development (LDRD) programme; Office of Naval Research (ONR) [N00014-09-1-1103]; National Science Foundation [1041979]; National Nuclear Security Administration of the US Department of Energy [DE-AC52-06NA25396] FX We acknowledge partial support from the Los Alamos National Laboratory's Laboratory Directed Research and Development (LDRD) programme and the Office of Naval Research (ONR) grant N00014-09-1-1103. This work was performed, in part, at the Center for Integrated Nanotechnologies, a user facility of the Office of Basic Energy Sciences. Los Alamos National Laboratory, an affirmative action equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the US Department of Energy under contract DE-AC52-06NA25396. BGP acknowledges the National Science Foundation for support though the American Competitiveness in Chemistry Fellowship (ACC-F) 1041979. NR 40 TC 13 Z9 13 U1 1 U2 40 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1367-2630 J9 NEW J PHYS JI New J. Phys. PD OCT 18 PY 2013 VL 15 AR 105016 DI 10.1088/1367-2630/15/10/105016 PG 12 WC Physics, Multidisciplinary SC Physics GA 236ML UT WOS:000325801200003 ER PT J AU Lin, WZ Li, Q Belianinov, A Sales, BC Sefat, A Gai, Z Baddorf, AP Pan, MH Jesse, S Kalinin, SV AF Lin, Wenzhi Li, Qing Belianinov, Alexei Sales, Brian C. Sefat, Athena Gai, Zheng Baddorf, Arthur P. Pan, Minghu Jesse, Stephen Kalinin, Sergei V. TI Local crystallography analysis for atomically resolved scanning tunneling microscopy images SO NANOTECHNOLOGY LA English DT Article ID FERROELECTRIC-FILMS; SURFACE; AU(111); SCALE AB Scanning probe microscopy has emerged as a powerful and flexible tool for atomically resolved imaging of surface structures. However, due to the amount of information extracted, in many cases the interpretation of such data is limited to being qualitative and semi-quantitative in nature. At the same time, much can be learned from local atom parameters, such as distances and angles, that can be analyzed and interpreted as variations of local chemical bonding, or order parameter fields. Here, we demonstrate an iterative algorithm for indexing and determining atomic positions that allows the analysis of inhomogeneous surfaces. This approach is further illustrated by local crystallographic analysis of several real surfaces, including highly ordered pyrolytic graphite and an Fe-based superconductor FeTe0:55Se0:45. This study provides a new pathway to extract and quantify local properties for scanning probe microscopy images. C1 [Lin, Wenzhi; Li, Qing; Belianinov, Alexei; Gai, Zheng; Baddorf, Arthur P.; Pan, Minghu; Jesse, Stephen; Kalinin, Sergei V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Sales, Brian C.; Sefat, Athena] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Lin, WZ (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM wenzhilinphysics@gmail.com; sergei2@ornl.gov RI Gai, Zheng/B-5327-2012; Kalinin, Sergei/I-9096-2012; Jesse, Stephen/D-3975-2016; Baddorf, Arthur/I-1308-2016; Sefat, Athena/R-5457-2016; OI Gai, Zheng/0000-0002-6099-4559; Kalinin, Sergei/0000-0001-5354-6152; Jesse, Stephen/0000-0002-1168-8483; Baddorf, Arthur/0000-0001-7023-2382; Sefat, Athena/0000-0002-5596-3504; Belianinov, Alex/0000-0002-3975-4112 FU Materials Sciences and Engineering Division, Office of Basic Energy Sciences, US Department of Energy; Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy FX Research for WL, BCS, AS and SVK was supported by the Materials Sciences and Engineering Division, Office of Basic Energy Sciences, US Department of Energy. This research was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. WSxM software has been used to assist the analysis [23]. NR 23 TC 1 Z9 1 U1 1 U2 24 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 J9 NANOTECHNOLOGY JI Nanotechnology PD OCT 18 PY 2013 VL 24 IS 41 AR 415707 DI 10.1088/0957-4484/24/41/415707 PG 6 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA 227UY UT WOS:000325141900020 PM 24060841 ER PT J AU Roberts, NA Gonzalez, CM Fowlkes, JD Rack, PD AF Roberts, Nicholas A. Gonzalez, Carlos M. Fowlkes, Jason D. Rack, Philip D. TI Enhanced by-product desorption via laser assisted electron beam induced deposition of W (CO)(6) with improved conductivity and resolution SO NANOTECHNOLOGY LA English DT Article ID CHEMICAL-VAPOR-DEPOSITION; TUNGSTEN HEXACARBONYL; FABRICATION; NANOSTRUCTURES; CRYSTALLIZATION; SUBSTRATE; NANOSCALE; W(CO)(6); FILMS AB Nanowires with higher tungsten (W) concentration and enhanced conductivity were grown via the laser assisted electron beam induced deposition (LAEBID) technique using tungsten hexacarbonyl W (CO)(6) as the gas precursor. Periodic, pulsed laser irradiation facilitated CO desorption during growth by heating the deposit. Deposit purity improved with laser pulse width up to the threshold for pyrolytic laser chemical vapor deposition (LCVD). Higher resolution was also observed and was attributed to reduced CO incorporation and higher deposit density. The optimal composition and lowest resistivity was achieved by synchronizing the electron beam induced deposition and laser assist such that (1) the electron beam induced deposit is less than a monolayer per cycle and (2) the laser induced heating is just below the LCVD threshold. C1 [Roberts, Nicholas A.] Utah State Univ, Dept Mech & Aerosp Engn, Logan, UT 84322 USA. [Gonzalez, Carlos M.; Rack, Philip D.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Fowlkes, Jason D.; Rack, Philip D.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Nanofabricat Res Lab, Oak Ridge, TN 37381 USA. RP Roberts, NA (reprint author), Utah State Univ, Dept Mech & Aerosp Engn, Logan, UT 84322 USA. EM prack@utk.edu RI Roberts, Nicholas/H-3275-2014; OI Roberts, Nicholas/0000-0002-6490-9454; Rack, Philip/0000-0002-9964-3254 NR 49 TC 9 Z9 9 U1 1 U2 17 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 J9 NANOTECHNOLOGY JI Nanotechnology PD OCT 18 PY 2013 VL 24 IS 41 AR 415301 DI 10.1088/0957-4484/24/41/415301 PG 6 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA 227UY UT WOS:000325141900005 PM 24045701 ER PT J AU Glenn, TC Lance, SL Mckee, AM Webster, BL Emery, AM Zerlotini, A Oliveira, G Rollinson, D Faircloth, BC AF Glenn, Travis C. Lance, Stacey L. Mckee, Anna M. Webster, Bonnie L. Emery, Aidan M. Zerlotini, Adhemar Oliveira, Guilherme Rollinson, David Faircloth, Brant C. TI Significant variance in genetic diversity among populations of Schistosoma haematobium detected using microsatellite DNA loci from a genome-wide database SO PARASITES & VECTORS LA English DT Article DE Africa; Differentiation; F-ST; Genomic; Microsatellites; Primer database; Schistosoma haematobium; Urogenital schistosomiasis ID UROGENITAL SCHISTOSOMIASIS; IMPLEMENTATION; SEQUENCES; MARKERS; PCR; DIFFERENTIATION; CONSERVATION; COLLECTION; INFECTION; SOFTWARE AB Background: Urogenital schistosomiasis caused by Schistosoma haematobium is widely distributed across Africa and is increasingly being targeted for control. Genome sequences and population genetic parameters can give insight into the potential for population-or species-level drug resistance. Microsatellite DNA loci are genetic markers in wide use by Schistosoma researchers, but there are few primers available for S. haematobium. Methods: We sequenced 1,058,114 random DNA fragments from clonal cercariae collected from a snail infected with a single Schistosoma haematobium miracidium. We assembled and aligned the S. haematobium sequences to the genomes of S. mansoni and S. japonicum, identifying microsatellite DNA loci across all three species and designing primers to amplify the loci in S. haematobium. To validate our primers, we screened 32 randomly selected primer pairs with population samples of S. haematobium. Results: We designed > 13,790 primer pairs to amplify unique microsatellite loci in S. haematobium, (available at http://www.cebio.org/projetos/schistosoma-haematobium-genome). The three Schistosoma genomes contained similar overall frequencies of microsatellites, but the frequency and length distributions of specific motifs differed among species. We identified 15 primer pairs that amplified consistently and were easily scored. We genotyped these 15 loci in S. haematobium individuals from six locations: Zanzibar had the highest levels of diversity; Malawi, Mauritius, Nigeria, and Senegal were nearly as diverse; but the sample from South Africa was much less diverse. Conclusions: About half of the primers in the database of Schistosoma haematobium microsatellite DNA loci should yield amplifiable and easily scored polymorphic markers, thus providing thousands of potential markers. Sequence conservation among S. haematobium, S. japonicum, and S. mansoni is relatively high, thus it should now be possible to identify markers that are universal among Schistosoma species (i.e., using DNA sequences conserved among species), as well as other markers that are specific to species or species-groups (i.e., using DNA sequences that differ among species). Full genome-sequencing of additional species and specimens of S. haematobium, S. japonicum, and S. mansoni is desirable to better characterize differences within and among these species, to develop additional genetic markers, and to examine genes as well as conserved non-coding elements associated with drug resistance. C1 [Glenn, Travis C.; Mckee, Anna M.] Univ Georgia, Dept Environm Hlth Sci, Athens, GA 30602 USA. [Lance, Stacey L.] Univ Georgia, Savannah River Ecol Lab, Aiken, SC 29802 USA. [Mckee, Anna M.] Univ Georgia, Warnell Sch Forestry & Nat Resources, Athens, GA 30602 USA. [Webster, Bonnie L.; Emery, Aidan M.; Rollinson, David] Wolfson Wellcome Biomed Labs, Dept Life Sci, Nat Hist Museum, London SW7 5BD, England. [Zerlotini, Adhemar; Oliveira, Guilherme] Fundacao Oswaldo Cruz, Natl Inst Sci & Technol Trop Dis, Rene Rachou Res Ctr, BR-30190002 Belo Horizonte, MG, Brazil. [Faircloth, Brant C.] Univ Calif Los Angeles, Dept Ecol & Evolut Biol, Los Angeles, CA 90095 USA. RP Glenn, TC (reprint author), Univ Georgia, Dept Environm Hlth Sci, Athens, GA 30602 USA. EM travisg@uga.edu RI Oliveira, Guilherme/E-2624-2014; Zerlotini, Adhemar/E-6533-2012; Lance, Stacey/K-9203-2013; Rollinson, David/C-7406-2009; OI Oliveira, Guilherme/0000-0003-0054-3438; Zerlotini, Adhemar/0000-0002-7739-0284; Lance, Stacey/0000-0003-2686-1733; Emery, Aidan/0000-0001-9028-8586; Faircloth, Brant/0000-0002-1943-0217 FU University of Georgia Research Foundation [RR374-053/0785426]; Bill & Melinda Gates Foundation [50816]; DOE [DEFC09-07SR22506] FX All researchers are grateful for the sub-awards (no. RR374-053/0785426) from the University of Georgia Research Foundation, which is awarded by the Bill & Melinda Gates Foundation (prime award no. 50816). Moreover they are particularly indebted to all members of the SCORE secretariat for valuable advice and input. We thank the Ministry of Health Zanzibar for collaboration and help with the isolation of parasites. We also thank the staff of the Georgia Genomics Facility for 454 DNA sequencing services. Manuscript preparation was partially supported by the DOE under Award Number DEFC09-07SR22506 to the University of Georgia Research Foundation. The authors would like to thank everyone that was involved in any of the field and NHM SCAN collections of the samples used in this study. We also thank Mike Anderson and Jayne King for their work in maintaining samples in the laboratory. NR 55 TC 9 Z9 9 U1 0 U2 19 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1756-3305 J9 PARASITE VECTOR JI Parasites Vectors PD OCT 17 PY 2013 VL 6 AR 300 DI 10.1186/1756-3305-6-300 PG 12 WC Parasitology SC Parasitology GA 277NX UT WOS:000328827400001 PM 24499537 ER PT J AU Peng, JK Ahluwalia, RK AF Peng, J. K. Ahluwalia, R. K. TI Enhanced dormancy due to para-to-ortho hydrogen conversion in insulated cryogenic pressure vessels for automotive applications SO INTERNATIONAL JOURNAL OF HYDROGEN ENERGY LA English DT Article DE Cryogenic hydrogen storage; Cryo-compressed tanks; Dormancy; Hydrogen loss; Para-to-ortho conversion ID STORAGE; VEHICLES; LIQUID AB A dynamic model has been developed to characterize dormancy and hydrogen loss from an insulated cryogenic pressure vessel that is filled with 99.79%-para liquid hydrogen to reach supercritical conditions. The model considers the thermodynamics and kinetics of the endothermic para-to-ortho conversion that occurs when the stored H-2 heats after the vessel is exposed to ambient conditions for an extended time. The thermal, thermodynamic, and kinetic aspects of the model were validated against experimental data obtained on a 151-L tank designed for service at nominal pressures up to 350 bar. Depending on the initial pressure, temperature, amount of H-2, and the rate of heat gain from the ambient, the endothermic para-to-ortho conversion can extend the loss-free dormancy time by up to 85%. Under conditions in which the endothermic conversion does not materially affect dormancy, it can still significantly reduce the H-2 loss rate and it can even introduce a secondary dormancy period. Copyright (C) 2013, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved. C1 [Peng, J. K.; Ahluwalia, R. K.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Ahluwalia, RK (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. EM walia@anl.gov FU Fuel Cell Technologies Office of the U.S. Department of Energy's (DOE) Office of Energy Efficiency and Renewable Energy; U.S. Department of Energy Office of Science laboratory [DE-AC02-06CH11357] FX This work was supported by the Fuel Cell Technologies Office of the U.S. Department of Energy's (DOE) Office of Energy Efficiency and Renewable Energy. Ms. Grace Ordaz of DOE was the Technology Development Manager for this study. Argonne National Laboratory, a U.S. Department of Energy Office of Science laboratory, is operated by UChicago Argonne, LLC, under Contract No. DE-AC02-06CH11357. NR 14 TC 5 Z9 5 U1 0 U2 10 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-3199 EI 1879-3487 J9 INT J HYDROGEN ENERG JI Int. J. Hydrog. Energy PD OCT 17 PY 2013 VL 38 IS 31 BP 13664 EP 13672 DI 10.1016/j.ijhydene.2013.08.039 PG 9 WC Chemistry, Physical; Electrochemistry; Energy & Fuels SC Chemistry; Electrochemistry; Energy & Fuels GA 252JC UT WOS:000327000000021 ER PT J AU Abbas, E Abelev, B Adam, J Adamova, D Adare, AM Aggarwal, MM Rinella, GA Agnello, M Agocs, AG Agostinelli, A Ahammed, Z Ahmad, N Masoodi, AA Ahn, SA Ahn, SU Aimo, I Ajaz, M Akindinov, A Aleksandrov, D Alessandro, B Alici, A Alkin, A Avina, EA Alme, J Alt, T Altini, V Altinpinar, S Altsybeev, I Andrei, C Andronic, A Anguelov, V Anielski, J Anson, C Anticic, T Antinori, F Antonioli, P Aphecetche, L Appelshauser, H Arbor, N Arcelli, S Arend, A Armesto, N Arnaldi, R Aronsson, T Arsene, IC Arslandok, M Asryan, A Augustinus, A Averbeck, R Awes, TC Aysto, J Azmi, MD Bach, M Badala, A Baek, YW Bailhache, R Bala, R Baldisseri, A Pedrosa, FBD Ban, J Baral, RC Barbera, R Barile, F Barnafoldi, GG Barnby, LS Barret, V Bartke, J Basile, M Bastid, N Basu, S Bathen, B Batigne, G Batyunya, B Batzing, PC Baumann, C Bearden, IG Beck, H Behera, NK Belikov, I Bellini, F Bellwied, R Belmont-Moreno, E Bencedi, G Beole, S Berceanu, I Bercuci, A Berdnikov, Y Berenyi, D Bergognon, AAE Bertens, RA Berzano, D Betev, L Bhasin, A Bhati, AK Bhom, J Bianchi, N Bianchi, L Bianchin, C Bielcik, J Bielcikova, J Bilandzic, A Bjelogrlic, S Blanco, F Blanco, F Blau, D Blume, C Boccioli, M Bottger, S Bogdanov, A Boggild, H Bogolyubsky, M Boldizsar, L Bombara, M Book, J Borel, H Borissov, A Bossu, F Botje, M Botta, E Braidot, E Braun-Munzinger, P Bregant, M Breitner, T Broker, TA Browning, TA Broz, M Brun, R Bruna, E Bruno, GE Budnikov, D Buesching, H Bufalino, S Buncic, P Busch, O Buthelezi, Z Caffarri, D Cai, X Caines, H Villar, EC Camerini, P Roman, VC Romeo, GC Carena, W Carena, F Carlin, N Carminati, F Diaz, AC Castellanos, JC Hernandez, JFC Casula, EAR Catanescu, V Cavicchioli, C Sanchez, CC Cepila, J Cerello, P Chang, B Chapeland, S Charvet, JL 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CA ALICE Collaboration TI J/psi Elliptic Flow in Pb-Pb Collisions at root s(NN)=2.76 TeV SO PHYSICAL REVIEW LETTERS LA English DT Article ID NUCLEAR COLLISIONS; SUPPRESSION; LHC AB We report on the first measurement of inclusive J/psi elliptic flow v(2) in heavy-ion collisions at the LHC. The measurement is performed with the ALICE detector in Pb-Pb collisions at root s(NN) = 2.76 TeV in the rapidity range 2.5 < y < 4.0. The dependence of the J/psi v(2) on the collision centrality and on the J/psi transverse momentum is studied in the range 0 <= p(T) < 10 GeV/c. For semicentral Pb-Pb collisions at root s(NN) = 2.76 TeV, an indication of nonzero v(2) is observed with a largest measured value of v(2) = 0.116 +/-0.046(stat) +/- 0.029(syst) for J/psi in the transverse momentum range 2 <= p(T) < 4 GeV/c. 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A.] Univ Santiago de Compostela, IGFAE, Santiago De Compostela, Spain. [Awes, T. C.; Ganoti, P.; Silvermyr, D.] Oak Ridge Natl Lab, Oak Ridge, TN USA. [Aysto, J.; Chang, B.; Kalliokoski, T.; Kim, D. J.; Kral, J.; Krizek, F.; Loo, K. K.; Morreale, A.; Raiha, T. S.; Rak, J.; Rasanen, S. S.; Sarkamo, J.; Trzaska, W. H.; Viinikainen, J.] HIP, Jyvaskyla, Finland. [Aysto, J.; Chang, B.; Kalliokoski, T.; Kim, D. J.; Kral, J.; Krizek, F.; Loo, K. K.; Morreale, A.; Raiha, T. S.; Rak, J.; Rasanen, S. S.; Sarkamo, J.; Trzaska, W. H.; Viinikainen, J.] Univ Jyvaskyla, Jyvaskyla, Finland. [Azmi, M. D.; Bossu, F.; Buthelezi, Z.; Clcymans, J.; Foertsch, S.; Murray, S.; Steyn, G.; Vilakazi, Z.] Univ Cape Town, Dept Phys, Somerset West, South Africa. [Azmi, M. D.; Bossu, F.; Buthelezi, Z.; Clcymans, J.; Foertsch, S.; Murray, S.; Steyn, G.; Vilakazi, Z.] Natl Res Fdn, iThemba LABS, Somerset West, South Africa. [Badala, A.; Palmeri, A.; Pappalardo, G. 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K.] Inst Phys, Bhubaneswar 751007, Orissa, India. [Barbera, R.; Jacholkowski, A.; La Rocca, P.; Petta, C.; Riggi, F.; Santagati, G.] Univ & Sez INFN, Dipartimento Fis & Astron, Catania, Italy. [Barnby, L. S.; Evans, D.; Hanratty, L. D.; Jones, P. G.; Jusko, A.; Krivda, M.; Lee, G. R.; Lietava, R.; Palaha, A.; Petrov, P.; Scott, P. A.; Baillie, O. Villalobos] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Bartke, J.; Figiel, J.; Gladysz-Dziadus, E.; Kowalski, M.; Matyja, A.; Mayer, C.; Rybicki, A.; Sputowska, I.; Szczepankiewicz, A.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Batyunya, B.; Grigoryan, S.; Malinina, L.; Mikhaylov, K.; Nomokonov, P.; Pocheptsov, T.; Rogochaya, E.; Shabratova, G.; Vala, M.; Vodopyanov, A.; Zaporozhets, S.] Joint Inst Nucl Res, Dubna, Russia. [Batzing, P. C.; Dordic, O.; Eyyubova, G.; Kvaerno, H.; Lindal, S.; Lovhoiden, G.; Milosevic, J.; Nilsson, M. S.; Qvigstad, H.; Richter, M.; Roed, K.; Skaali, T. 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RI Akindinov, Alexander/J-2674-2016; Nattrass, Christine/J-6752-2016; Suaide, Alexandre/L-6239-2016; Deppman, Airton/J-5787-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Ferreiro, Elena/C-3797-2017; Armesto, Nestor/C-4341-2017; Ferretti, Alessandro/F-4856-2013; Martinez Hernandez, Mario Ivan/F-4083-2010; Vickovic, Linda/F-3517-2017; Fernandez Tellez, Arturo/E-9700-2017; Graczykowski, Lukasz/O-7522-2015; Janik, Malgorzata/O-7520-2015; feofilov, grigory/A-2549-2013; Adamova, Dagmar/G-9789-2014; Christensen, Christian/D-6461-2012; De Pasquale, Salvatore/B-9165-2008; Chinellato, David/D-3092-2012; de Cuveland, Jan/H-6454-2016; Kurepin, Alexey/H-4852-2013; Jena, Deepika/P-2873-2015; Jena, Satyajit/P-2409-2015; Salgado, Carlos A./G-2168-2015; Bruna, Elena/C-4939-2014; Karasu Uysal, Ayben/K-3981-2015; HAMAGAKI, HIDEKI/G-4899-2014; Pshenichnov, Igor/A-4063-2008; Kompaniets, Mikhail/F-5025-2013; Altsybeev, Igor/K-6687-2013; Vinogradov, Leonid/K-3047-2013; Kondratiev, Valery/J-8574-2013; Vechernin, Vladimir/J-5832-2013; Zarochentsev, Andrey/J-6253-2013; Barnby, Lee/G-2135-2010; Blau, Dmitry/H-4523-2012; Yang, Hongyan/J-9826-2014; Cosentino, Mauro/L-2418-2014; Bearden, Ian/M-4504-2014; Sumbera, Michal/O-7497-2014; Felea, Daniel/C-1885-2012; Barnafoldi, Gergely Gabor/L-3486-2013; Peitzmann, Thomas/K-2206-2012; Kharlov, Yuri/D-2700-2015; Mitu, Ciprian/E-6733-2011; Usai, Gianluca/E-9604-2015; Castillo Castellanos, Javier/G-8915-2013; Levai, Peter/A-1544-2014; Pochybova, Sona/A-2835-2014; Krizek, Filip/G-8967-2014; Bielcikova, Jana/G-9342-2014; Takahashi, Jun/B-2946-2012; Kovalenko, Vladimir/C-5709-2013; Guber, Fedor/I-4271-2013; Bregant, Marco/I-7663-2012; Wagner, Vladimir/G-5650-2014; Sevcenco, Adrian/C-1832-2012; Kucera, Vit/G-8459-2014; Vajzer, Michal/G-8469-2014 OI Akindinov, Alexander/0000-0002-7388-3022; Nattrass, Christine/0000-0002-8768-6468; Suaide, Alexandre/0000-0003-2847-6556; Deppman, Airton/0000-0001-9179-6363; Ferreiro, Elena/0000-0002-4449-2356; Armesto, Nestor/0000-0003-0940-0783; Ferretti, Alessandro/0000-0001-9084-5784; Martinez Hernandez, Mario Ivan/0000-0002-8503-3009; Vickovic, Linda/0000-0002-9820-7960; Fernandez Tellez, Arturo/0000-0003-0152-4220; Janik, Malgorzata/0000-0002-3356-3438; feofilov, grigory/0000-0003-3700-8623; Christensen, Christian/0000-0002-1850-0121; De Pasquale, Salvatore/0000-0001-9236-0748; Chinellato, David/0000-0002-9982-9577; de Cuveland, Jan/0000-0003-0455-1398; Kurepin, Alexey/0000-0002-1851-4136; Jena, Deepika/0000-0003-2112-0311; Jena, Satyajit/0000-0002-6220-6982; Salgado, Carlos A./0000-0003-4586-2758; Bruna, Elena/0000-0001-5427-1461; Karasu Uysal, Ayben/0000-0001-6297-2532; Pshenichnov, Igor/0000-0003-1752-4524; Kompaniets, Mikhail/0000-0001-8831-0553; Altsybeev, Igor/0000-0002-8079-7026; Vinogradov, Leonid/0000-0001-9247-6230; Kondratiev, Valery/0000-0002-0031-0741; Vechernin, Vladimir/0000-0003-1458-8055; Zarochentsev, Andrey/0000-0002-3502-8084; Barnby, Lee/0000-0001-7357-9904; Cosentino, Mauro/0000-0002-7880-8611; Bearden, Ian/0000-0003-2784-3094; Sumbera, Michal/0000-0002-0639-7323; Felea, Daniel/0000-0002-3734-9439; Peitzmann, Thomas/0000-0002-7116-899X; Usai, Gianluca/0000-0002-8659-8378; Castillo Castellanos, Javier/0000-0002-5187-2779; Takahashi, Jun/0000-0002-4091-1779; Kovalenko, Vladimir/0000-0001-6012-6615; Guber, Fedor/0000-0001-8790-3218; Sevcenco, Adrian/0000-0002-4151-1056; FU State Committee of Science; World Federation of Scientists (WFS); Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq); Financiadora de Estudos e Projetos (FINEP); Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC); Chinese Ministry of Education (CMOE); Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council; Carlsberg Foundation; Danish National Research Foundation; European Research Council under the European Community; Helsinki Institute of Physics; Academy of Finland; French CNRS-IN2P3; Region Pays de Loire; Region Alsace; Region Auvergne; CEA, France; German BMBF; Helmholtz Association; General Secretariat for Research and Technology; Ministry of Development, Greece; Hungarian OTKA; National Office for Research and Technology (NKTH); Department of Atomic Energy; Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN); Centro Fermi-Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi," Italy; MEXT, Japan; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); CONACYT; DGAPA, Mexico; ALFA-EC; EPLANET Program (European Particle Physics Latin American Network); Stichting voor Fundamenteel Onderzoek der Materie (FOM); Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); Polish Ministry of Science and Higher Education; National Authority for Scientific Research-NASR (Autoritatea Nationala pentru Cercetare Stiintifica-ANCS); Ministry of Education and Science of Russian Federation; Russian Academy of Sciences; Russian Federal Agency of Atomic Energy; Russian Federal Agency for Science and Innovations; Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, South Africa; CIEMAT; EELA; Ministerio de Economia y Competitividad (MINECO) of Spain; Xunta de Galicia (Conselleria de Educacion); CEADEN; Cubaenergia, Cuba; IAEA (International Atomic Energy Agency); Swedish Research Council (VR); Knut & Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); U.S. Department of Energy; U.S. National Science Foundation; State of Texas; State of Ohio FX The ALICE Collaboration would like to thank all its engineers and technicians for their invaluable contributions to the construction of the experiment and the CERN accelerator teams for the outstanding performance of the LHC complex. The ALICE Collaboration acknowledges the following funding agencies for their support in building and running the ALICE detector: State Committee of Science, World Federation of Scientists (WFS) and Swiss Fonds Kidagan, Armenia, Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq), Financiadora de Estudos e Projetos (FINEP), Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC), the Chinese Ministry of Education (CMOE), and the Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council, the Carlsberg Foundation, and the Danish National Research Foundation; The European Research Council under the European Community's Seventh Framework Programme; Helsinki Institute of Physics and the Academy of Finland; French CNRS-IN2P3, the "Region Pays de Loire," "Region Alsace," " Region Auvergne," and CEA, France; German BMBF and the Helmholtz Association; General Secretariat for Research and Technology, Ministry of Development, Greece; Hungarian OTKA and National Office for Research and Technology (NKTH); Department of Atomic Energy and Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN) and Centro Fermi-Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi," Italy; MEXT Grant-in-Aid for Specially Promoted Research, Japan; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); CONACYT, DGAPA, Mexico, ALFA-EC, and the EPLANET Program (European Particle Physics Latin American Network); Stichting voor Fundamenteel Onderzoek der Materie (FOM) and the Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); Polish Ministry of Science and Higher Education; National Authority for Scientific Research-NASR (Autoritatea Nationala pentru Cercetare Stiintifica-ANCS); Ministry of Education and Science of Russian Federation, Russian Academy of Sciences, Russian Federal Agency of Atomic Energy, Russian Federal Agency for Science and Innovations, and The Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, South Africa; CIEMAT, EELA, Ministerio de Economia y Competitividad (MINECO) of Spain, Xunta de Galicia (Conselleria de Educacion), CEADEN, Cubaenergia, Cuba, and IAEA (International Atomic Energy Agency); Swedish Research Council (VR) and Knut & Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); U.S. Department of Energy, U.S. National Science Foundation, the State of Texas, and the State of Ohio. NR 29 TC 31 Z9 31 U1 0 U2 94 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 17 PY 2013 VL 111 IS 16 AR 162301 DI 10.1103/PhysRevLett.111.162301 PG 11 WC Physics, Multidisciplinary SC Physics GA 241DY UT WOS:000326147800005 PM 24182258 ER PT J AU El Hedri, S Hook, A AF El Hedri, Sonia Hook, Anson TI Minimal signatures of naturalness SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Supersymmetry Phenomenology; Phenomenology of Large extra dimensions ID MODEL HIGGS-BOSON; ATLAS DETECTOR; ROOT-S=7 TEV; HIERARCHY PROBLEM; PP COLLISIONS; SEARCH; LHC AB We study the naturalness problem using a model independent bottom up approach by considering models where only the interaction terms needed to cancel the Higgs quadratic divergences are present. If quadratic divergences are canceled by terms linear in the Higgs field, then the collider phenomenology is well covered by current electroweakino and fourth generation searches. If quadratic divergences are canceled by terms bilinear in the Higgs field, then the signatures are highly dependent on the quantum numbers of the new particles. Precision Higgs measurements can reveal the presence of new particles with either vevs or Standard Model charges. If the new particles are scalar dark matter candidates, their direct and indirect detection signatures will be highly correlated and within the reach of XENON100 and Fermi. Observation at one of these experiments would imply observation at the other one. Observable LHC decay channels can also arise if the new particles mix with lighter states. This decay channel involves only the Higgs boson and not the gauge bosons. Observation of such decays would give evidence that the new particle is tied to the naturalness problem. C1 [El Hedri, Sonia] Stanford Univ, SLAC, Menlo Pk, CA 94025 USA. [Hook, Anson] Princeton Univ, Inst Adv Studies, Princeton, NJ 08540 USA. RP El Hedri, S (reprint author), Stanford Univ, SLAC, Sand Hill Rd, Menlo Pk, CA 94025 USA. EM soniaeh@slac.stanford.edu; hook@ias.edu FU Stanford Graduate Fellowship; US DOE [DE-FG02-90ER40542] FX The authors would like to thank Tim Cohen, Nathaniel Craig, Mariangela Lisanti and Jay Wacker for helpful discussions. The authors would also like to thank Tim Cohen and Mariangela Listanti for comments on the draft. SE is supported by a Stanford Graduate Fellowship. AH is supported by the US DOE under contract number DE-FG02-90ER40542. NR 63 TC 3 Z9 3 U1 0 U2 2 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD OCT 17 PY 2013 IS 10 AR 105 DI 10.1007/JHEP10(2013)105 PG 26 WC Physics, Particles & Fields SC Physics GA 236RZ UT WOS:000325818200004 ER PT J AU Koenig, GM Ma, JW Key, B Fink, J Low, KB Shahbazian-Yassar, R Belharouak, I AF Koenig, Gary M., Jr. Ma, Jiwei Key, Baris Fink, Justin Low, Ke-Bin Shahbazian-Yassar, Reza Belharouak, Ilias TI Composite of LiFePO4 with Titanium Phosphate Phases as Lithium-Ion Battery Electrode Material SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID ELECTROCHEMICAL PROPERTIES; CATHODE MATERIALS; CONDUCTIVITY; POWER AB We report the synthesis of LiFePO4 (LFP) battery materials where during synthesis the iron has been substituted by up to 10 mol % with titanium. Analysis of the Ti-substituted materials revealed that at the substitution levels investigated, the Ti did not form a solid solution with the LFP, but rather minority phases containing Ti phosphates were formed and segregated at the nanoscopic scale. The minority phases were amorphous or not well-crystallized and accepted Li on first discharge in a lithium half cell, and solid state NMR spectra were consistent with one of the constituents being LiTi2(PO4)(3). The Ti substituted materials had increased electrochemical capacities and discharge voltages relative to LFP prepared in an equivalent process, and the ability to accept Li on first discharge may find utility in using previously inaccessible capacity in battery cathode formulations and in balancing excess capacity from high energy cathode materials. C1 [Koenig, Gary M., Jr.; Ma, Jiwei; Key, Baris; Fink, Justin; Belharouak, Ilias] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Low, Ke-Bin; Shahbazian-Yassar, Reza] Univ Illinois, Res Resources Ctr East MC 337, Chicago, IL 60607 USA. [Shahbazian-Yassar, Reza] Michigan Technol Univ, Dept Mech Engn, Houghton, MI 49931 USA. RP Belharouak, I (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM gary.koenig@virginia.edu; belharouak@anl.gov OI Belharouak, Ilias/0000-0002-3985-0278 FU U.S. Department of Energy, Freedom CAR, and Vehicle Technologies Office; U.S. Department of Energy by UChicago Argonne, LLC [DE-ACOZ-06CH11357] FX This research was funded by the U.S. Department of Energy, Freedom CAR, and Vehicle Technologies Office. The electron microscopy was accomplished at the Electron Microscopy Center for Materials Research at Argonne National Laboratory, a U.S. Department of Energy Office of Science Laboratory. Argonne National Laboratory is operated for the U.S. Department of Energy by UChicago Argonne, LLC, under Contract DE-ACOZ-06CH11357. NR 29 TC 4 Z9 4 U1 9 U2 52 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 EI 1932-7455 J9 J PHYS CHEM C JI J. Phys. Chem. C PD OCT 17 PY 2013 VL 117 IS 41 BP 21132 EP 21138 DI 10.1021/jp4074174 PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 240VM UT WOS:000326125800012 ER PT J AU Cui, GF Liu, SF Zhao, J Holby, EF Li, Q Wu, G AF Cui, Guofeng Liu, Shaofang Zhao, Jie Holby, Edward F. Li, Qing Wu, Gang TI AuSn20 Eutectic Electrodeposition through Alternative Complexing of Pyrophosphoric Acid: Insights from Electrochemical and DFT Methods SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID EFFECTIVE CORE POTENTIALS; ELECTROLESS DEPOSITION PROCESS; AU-SN ALLOY; MOLECULAR CALCULATIONS; DIMETHYLAMINE BORANE; INTERFACIAL REACTION; OXIDATION MECHANISM; DENSITY; SOLDER; REDUCTANT AB Eutectic AuSn20 solder is an important material for electronic packaging technology due to its superior mechanical and thermal conductive properties. In this work, AuSn20 alloy films are prepared via the electrodeposition method for the first time. The electrodeposition is cost-effective with improved control over the alloy content when compared to traditional powdered metallurgy methods. Pyrophosphoric acid was found to be an effective complexing agent to minimize the difference of the deposition potentials between Au and Sn, making the codeposition of AuSn alloys possible. Importantly, electrochemical characterization was combined with density functional theory (DFT) calculations to provide insight into the mechanism of the alloy codeposition when pyrophosphoric acid was used as the complexing agent. In particular, natural bond orbital (NBO) charge distribution and the lowest unoccupied molecular orbital (LUMO) characteristics of [P2O7](4-)-Sn(II) and [P2O7](4-)-Au(I) complexes are calculated, suggesting that [P2O7](4-) is able to coordinate more strongly with Sn(II) than Au(I). As a result, it can thus shift the deposition potentials of Au(I) and Sn(II) much closer. As the DFT predicted, the role of pyrophosphoric acid as a complexing agent has been experimentally verified, making codeposition of Au and Sn realistic. The structures of the obtained AuSn20 films are determined using scanning electron microscopy (SEM) and energy dispersive X-ray spectrometry (EDX) and found to be consistent with AuSn/Au5Sn eutectic as predicted by the Au-Sn phase diagram. Additionally, the measured melting point is in good agreement with the theoretically determined one. Relevant tests demonstrated in this work indicate that the newly developed electrodeposited AuSn20 alloy coatings are suitable for microelectronic soldering applications. C1 [Cui, Guofeng; Liu, Shaofang] Sun Yat Sen Univ, Sch Chem & Chem Engn, Key Lab Low Carbon Chem & Energy Conservat Guangd, Guangzhou 510275, Guangdong, Peoples R China. [Zhao, Jie] S China Univ Technol, Sch Mech & Automot Engn, Guangzhou 510640, Guangdong, Peoples R China. [Holby, Edward F.; Li, Qing; Wu, Gang] Los Alamos Natl Lab, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA. RP Cui, GF (reprint author), Sun Yat Sen Univ, Sch Chem & Chem Engn, Key Lab Low Carbon Chem & Energy Conservat Guangd, Guangzhou 510275, Guangdong, Peoples R China. EM cuigf@mail.sysu.edu.cn RI Wu, Gang/E-8536-2010; Li, Qing/G-4502-2011; OI Wu, Gang/0000-0003-4956-5208; Li, Qing/0000-0003-4807-030X; Holby, Edward/0000-0001-8419-6298 FU National Natural Science Foundation of China [51271205, 50801070]; Fundamental Research Funds for the Central Universities [11lgpy08]; Guangzhou Pearl Technology the Nova Special Project [2012J2200058]; Research and Application of Key Technologies Oriented the Industrial Development [90035-3283309]; "Plan of Science and Technology Project" by the DaYa Gulf district in Huizhou city [31000-4207387]; Innovative Laboratory Fund by Sun Yat-Sen University FX G.F.C. gratefully acknowledges the financial support by National Natural Science Foundation of China (51271205, 50801070), "The Fundamental Research Funds for the Central Universities" (11lgpy08), "Guangzhou Pearl Technology the Nova Special Project" (2012J2200058), "Research and Application of Key Technologies Oriented the Industrial Development" (90035-3283309), "Plan of Science and Technology Project" by the DaYa Gulf district in Huizhou city (31000-4207387), and the Innovative Laboratory Fund by Sun Yat-Sen University. NR 29 TC 2 Z9 2 U1 2 U2 43 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 EI 1932-7455 J9 J PHYS CHEM C JI J. Phys. Chem. C PD OCT 17 PY 2013 VL 117 IS 41 BP 21228 EP 21233 DI 10.1021/jp408721e PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 240VM UT WOS:000326125800022 ER PT J AU Bardhan, R Zarick, HF Schwartzberg, A Pint, CL AF Bardhan, Rizia Zarick, Holly F. Schwartzberg, Adam Pint, Cary L. TI Size-Dependent Phononic Properties of PdO Nanocrystals Probed by Nanoscale Optical Thermometry SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID TRANSITION-METAL OXIDES; THERMAL-CONDUCTIVITY; RAMAN-SPECTROSCOPY; SILICON NANOWIRES; NANOSTRUCTURED MATERIALS; HIGHLY EFFICIENT; THIN-FILMS; OXIDATION; CATALYSTS; SEMICONDUCTOR AB With the advent of novel nanoscale devices, fast and reliable thermal mapping with high spatiotemporal resolution is imperative for probing the characteristics of phonons and evaluating the local temperature at the nanoscale. In this work, Raman spectroscopy is employed as a rapid and noncontact optical thermometry technique to investigate phononic properties of macroscopic assemblies of monodisperse palladium oxide (PdO) nanocrystals. PdO has been extensively employed in high temperature catalytic devices; however, the phonon behavior which determines the thermal stability of PdO remains unexplored thus far. Our study focuses on homogeneous, large-scale assemblies of monodisperse 4 and 10 nm nanocrystals synthesized using colloidal chemistry to understand size-dependent effects on the measured thermal properties. By monitoring the Raman peak shifts, peak broadening, and alterations in peak intensities as a function of laser power and particle concentration, a size-dependent trend is observed attributable to confinement of optical phonons within nanocrystal grain boundaries and laser-induced heating, both influenced by nanocrystal size. This study correlates size-dependent single-particle heating effects with size-dependent interparticle heat transfer under laser irradiation and is enabled by controlled nanocrystal synthesis. C1 [Bardhan, Rizia; Zarick, Holly F.] Vanderbilt Univ, Dept Chem & Biomol Engn, Nashville, TN 37235 USA. [Schwartzberg, Adam] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Mol Foundry, Berkeley, CA 94720 USA. [Pint, Cary L.] Vanderbilt Univ, Dept Mech Engn, Nashville, TN 37235 USA. RP Bardhan, R (reprint author), Vanderbilt Univ, Dept Chem & Biomol Engn, 221 Kirkland Hall, Nashville, TN 37235 USA. EM rizia.bardhan@vanderbilt.edu RI Bardhan, Rizia/B-4674-2014; Pint, Cary/I-6785-2013 FU Vanderbilt start-up funds; NSF-EPSCoR [EPS1004083]; Department of Education [P200A090323]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX This work was supported by Vanderbilt start-up funds and NSF-EPSCoR (EPS1004083). HFZ acknowledges support from the Department of Education for a Graduate Assistance in Areas of National Need (GAANN) Fellowship under grant number P200A090323. Characterization aspects of this research were conducted in part at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. NR 77 TC 3 Z9 3 U1 2 U2 38 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 EI 1932-7455 J9 J PHYS CHEM C JI J. Phys. Chem. C PD OCT 17 PY 2013 VL 117 IS 41 BP 21558 EP 21568 DI 10.1021/jp406916h PG 11 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 240VM UT WOS:000326125800058 ER PT J AU El-Khoury, PZ Hu, DH Hess, WP AF El-Khoury, Patrick Z. Hu, Dehong Hess, Wayne P. TI Junction Plasmon-Induced Molecular Reorientation SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID ENHANCED RAMAN-SPECTROSCOPY; SCATTERING AB Time- and frequency-dependent intensity variations in sequences of Raman spectra recorded at plasmonic junctions can be assigned to molecular reorientation. This is revealed through Raman trajectories recorded at a nanojunction formed between a silver atomic force microscope tip and a corrugated silver surface coated with biphenyl-4,4'-dithiol. Molecular motion is not observed when the tip is retracted, and only surface enhancement is operative. In effect, junction plasmon-induced molecular reorientation is tracked. C1 [El-Khoury, Patrick Z.; Hu, Dehong; Hess, Wayne P.] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. RP El-Khoury, PZ (reprint author), Pacific NW Natl Lab, Div Phys Sci, POB 999, Richland, WA 99352 USA. EM patrick.elkhoury@pnnl.gov; wayne.hess@pnnl.gov RI Hu, Dehong/B-4650-2010 OI Hu, Dehong/0000-0002-3974-2963 FU U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences Biosciences; Laboratory Directed Research and Development Program through a Linus Pauling Fellowship at Pacific Northwest National Laboratory (PNNL); DOE's Office of Biological and Environmental Research FX W.P.H. acknowledges support from the U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences & Biosciences. P.Z.E. acknowledges support from the Laboratory Directed Research and Development Program through a Linus Pauling Fellowship at Pacific Northwest National Laboratory (PNNL), an allocation of computing time from the National Science Foundation (TG-CHE130003), and the use of the Extreme Science and Engineering Discovery Environment. This work was performed using EMSL, a national scientific user facility sponsored by the DOE's Office of Biological and Environmental Research and located at PNNL. PNNL is a multiprogram national laboratory operated for DOE by Battelle. NR 18 TC 12 Z9 12 U1 0 U2 8 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD OCT 17 PY 2013 VL 4 IS 20 BP 3435 EP 3439 DI 10.1021/jz401838b PG 5 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 240UZ UT WOS:000326124500012 ER PT J AU Luntz, AC Viswanathan, V Voss, J Varley, JB Norskov, JK Scheffler, R Speidel, A AF Luntz, A. C. Viswanathan, V. Voss, J. Varley, J. B. Norskov, J. K. Scheffler, R. Speidel, A. TI Tunneling and Polaron Charge Transport through Li2O2 in Li-O-2 Batteries SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID LI-AIR BATTERIES; KINETIC OVERPOTENTIALS; LITHIUM; LIMITATIONS AB We describe Li-O-2 discharge experiments in a bulk electrolysis cell as a function of current density and temperature. In combination with a simple model, these imply that charge transport through Li2O2 in Li-O-2 batteries at practical current densities is based principally on hole tunneling, with hole polaron conductivity playing a significant role near the end of very low current discharges and at temperatures greater than 30 degrees C. We also show that charge-transport limitations are much less significant during charging than those in discharge. A key element of the model that qualitatively explains all results is the alignment of the Li2O2 valence band maximum close to the electrochemical Fermi energy and how this alignment varies with overpotentials during discharge and charge. In fact, comparison of the model with the experiments allows determination of the alignment of the bands relative to the electrochemical Fermi level. C1 [Luntz, A. C.] IBM Res Corp, Almaden Res Ctr, San Jose, CA 95120 USA. [Luntz, A. C.; Viswanathan, V.; Voss, J.; Varley, J. B.; Norskov, J. K.] SLAC Natl Accelerator Lab, SUNCAT, Menlo Pk, CA 94025 USA. [Viswanathan, V.; Norskov, J. K.] Stanford Univ, Dept Chem Engn, Stanford, CA 94305 USA. [Scheffler, R.; Speidel, A.] Volkswagen Grp Inc, Belmont, CA 94002 USA. [Varley, J. B.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Luntz, AC (reprint author), IBM Res Corp, Almaden Res Ctr, 650 Harry Rd, San Jose, CA 95120 USA. EM acluntz@pacbell.net RI Norskov, Jens/D-2539-2017; OI Norskov, Jens/0000-0002-4427-7728; Viswanathan, Venkatasubramanian/0000-0003-1060-5495 FU U.S. Department of Energy, Chemical Sciences, Geosciences and Biosciences Division [DE-AC02-76SF00515]; ReLiable project [11-116792]; Danish Council for Strategic Research FX The authors acknowledge partial support of this work from the U.S. Department of Energy, Chemical Sciences, Geosciences and Biosciences Division under Contract Number DE-AC02-76SF00515 and the ReLiable project (# 11-116792) funded by The Danish Council for Strategic Research. We also wish to thank J. Hununelshoj, Don Siegel, and B. D. McCloskey for useful discussions. NR 17 TC 55 Z9 55 U1 5 U2 66 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD OCT 17 PY 2013 VL 4 IS 20 BP 3494 EP 3499 DI 10.1021/jz401926f PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 240UZ UT WOS:000326124500021 ER PT J AU Jin, SY DeMarco, E Pellin, MJ Farha, OK Wiederrecht, GP Hupp, JT AF Jin, Shengye DeMarco, Erica Pellin, Michael J. Farha, Omar K. Wiederrecht, Gary P. Hupp, Joseph T. TI Distance-Engineered Plasmon-Enhanced Light Harvesting in CdSe Quantum Dots SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID SENSITIZED SOLAR-CELLS; INTERFACIAL ELECTRON-TRANSFER; SINGLE-MOLECULE FLUORESCENCE; GOLD NANOPARTICLES; SEMICONDUCTOR NANOCRYSTALS; CHARGE SEPARATION; NANOROD HETEROSTRUCTURES; COLLOIDAL NANOCRYSTALS; HYDROGEN-PRODUCTION; ENERGY-TRANSFER AB Improvement of light harvesting in semiconductor quantum dots (QDs) is essential for the development of efficient QD-based solar energy conversion systems. In this study, plasmon-enhanced light absorption in CdSe QDs sensitized on silver (Ag) nanoparticle (NP) films was examined as a function of interparticle (QD to Ag NP) distance. Up to 24-fold plasmonic enhancement of fluorescence from QDs was observed when the particle separation distance was >= 5 nm. The enhancement effect was observed to largely sustain the exciton lifetimes in QDs and to strongly depend on the incident photon wavelength following the plasmon resonant strength of Ag NPs, confirming that the enhanced photoluminescence was mainly due to the enhancement in photoabsorption in CdSe QDs by the plasmon of Ag NPs. This study suggests applications of Ag NPs in QD-based solar energy conversion for significantly improving light harvesting in QDs. C1 [Jin, Shengye; Wiederrecht, Gary P.] Argonne Natl Lab, Nanosci & Technol Div, Argonne, IL 60439 USA. [Pellin, Michael J.; Hupp, Joseph T.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Hupp, Joseph T.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [DeMarco, Erica; Farha, Omar K.; Wiederrecht, Gary P.; Hupp, Joseph T.] Northwestern Univ, Argonne Northwestern Solar Energy Res Ctr, Evanston, IL 60208 USA. [Jin, Shengye; DeMarco, Erica; Pellin, Michael J.; Farha, Omar K.; Hupp, Joseph T.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. RP Wiederrecht, GP (reprint author), Argonne Natl Lab, Nanosci & Technol Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM wiederrecht@anl.gov RI Pellin, Michael/B-5897-2008 OI Pellin, Michael/0000-0002-8149-9768 FU Argonne-Northwestern Solar Energy Research (ANSER) Center, an Energy Frontier Research Center; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001059, DE-AC02-06CH11357] FX This work was supported as part of the Argonne-Northwestern Solar Energy Research (ANSER) Center, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Award Number DE-SC0001059. Use of the Center for Nanoscale Materials was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences through Contract No. DE-AC02-06CH11357. NR 63 TC 24 Z9 24 U1 8 U2 115 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD OCT 17 PY 2013 VL 4 IS 20 BP 3527 EP 3533 DI 10.1021/jz401801v PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 240UZ UT WOS:000326124500026 ER PT J AU Ahn, KH Seman, TF Lookman, T Bishop, AR AF Ahn, K. H. Seman, T. F. Lookman, T. Bishop, A. R. TI Role of complex energy landscapes and strains in multiscale inhomogeneities in perovskite manganites SO PHYSICAL REVIEW B LA English DT Article ID METAL-INSULATOR-TRANSITION; PHASE-SEPARATED MANGANITES; COLOSSAL-MAGNETORESISTANCE; MANGANESE PEROVSKITES; THIN-FILM; OXIDES; LA1-XSRXMNO3; RESISTIVITY; PERCOLATION; PHYSICS AB We analyze the essential role played by complex energy landscapes in the nanometer- to micron-scale inhomogeneities observed in perovskite manganites using a model expressed in terms of symmetrized atomic-scale lattice distortion modes. We also examine the stability of large metal and insulator domains in the absence of defects. Our results demonstrate that an intrinsic mechanism, which involves long-range interactions between strain fields, the Peierls-Nabarro energy barrier, and complex energy landscapes with multiple metastable states, rather than an extrinsic mechanism such as chemical randomness, is responsible for the inhomogeneity in perovskite manganites. C1 [Ahn, K. H.; Seman, T. F.] New Jersey Inst Technol, Dept Phys, Newark, NJ 07102 USA. [Lookman, T.; Bishop, A. R.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Ahn, KH (reprint author), New Jersey Inst Technol, Dept Phys, Newark, NJ 07102 USA. EM kenahn@njit.edu FU US DOE/LANL [DE-AC52-06NA25396/170590-1]; US DOE LANL LDRD FX We thank Avadh Saxena and Yoonseok Lee for discussions. This work has been supported by US DOE/LANL Award No. DE-AC52-06NA25396/170590-1 (T.F.S. and K.H.A.) and by US DOE LANL LDRD (T.L. and A.R.B.). NR 65 TC 4 Z9 4 U1 2 U2 29 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD OCT 17 PY 2013 VL 88 IS 14 AR 144415 DI 10.1103/PhysRevB.88.144415 PG 15 WC Physics, Condensed Matter SC Physics GA 240GC UT WOS:000326082000002 ER PT J AU Song, Y Regnault, LP Zhang, CL Tan, GT Carr, SV Chi, SX Christianson, AD Xiang, T Dai, PC AF Song, Yu Regnault, Louis-Pierre Zhang, Chenglin Tan, Guotai Carr, Scott V. Chi, Songxue Christianson, A. D. Xiang, Tao Dai, Pengcheng TI In-plane spin excitation anisotropy in the paramagnetic state of NaFeAs SO PHYSICAL REVIEW B LA English DT Article ID CA(FE1-XCOX)(2)AS-2; SUPERCONDUCTORS; TRANSITION AB We use unpolarized and polarized inelastic neutron scattering to study low-energy spin excitations in NaFeAs, which exhibits a tetragonal-to-orthorhombic lattice distortion at T-s approximate to 58 K followed by a collinear antiferromagnetic (AF) order below T-N approximate to 45 K. In the AF ordered state (T < T-N), spin waves are entirely c-axis polarized below similar to 10 meV, exhibiting a gap of similar to 4 meV at the AF zone center and disperse to similar to 7 meV near the c-axis AF zone boundary. On warming to the paramagnetic state with orthorhombic lattice distortion (T-N < T < T-s), spin excitations become anisotropic within the FeAs plane. Upon further warming to the paramagnetic tetragonal state (T > T-s), spin excitations become more isotropic. Since similar magnetic anisotropy is also observed in the paramagnetic tetragonal phase of superconducting BaFe1.904Ni0.096As2, our results suggest that the spin excitation anisotropy in superconducting iron pnictides originates from similar anisotropy already present in their parent compounds. C1 [Song, Yu; Zhang, Chenglin; Carr, Scott V.; Dai, Pengcheng] Rice Univ, Dept Phys & Astron, Houston, TX 77005 USA. [Song, Yu; Zhang, Chenglin; Tan, Guotai; Carr, Scott V.; Dai, Pengcheng] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Regnault, Louis-Pierre] CEA Grenoble, UJF Grenoble 1, INAC, SPSMS MDN,UMR E, F-38054 Grenoble, France. [Chi, Songxue; Christianson, A. D.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Xiang, Tao; Dai, Pengcheng] Chinese Acad Sci, Inst Phys, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China. RP Song, Y (reprint author), Rice Univ, Dept Phys & Astron, Houston, TX 77005 USA. EM pdai@rice.edu RI Dai, Pengcheng /C-9171-2012; christianson, andrew/A-3277-2016; Chi, Songxue/A-6713-2013 OI Song, Yu/0000-0002-3460-393X; Dai, Pengcheng /0000-0002-6088-3170; christianson, andrew/0000-0003-3369-5884; Chi, Songxue/0000-0002-3851-9153 FU US DOE, BES [DE-FG02-05ER46202]; MOST (973 Project) [2012CB82400]; Scientific User Facilities Division, BES, US DOE FX We thank Haifeng Li and T. Netherton for experimental assistance, and Jiangping Hu and Fa Wang for helpful discussions. The single crystal growth efforts and neutron scattering work at UTK and Rice are supported by the US DOE, BES, through Contract DE-FG02-05ER46202. Work at IOP is supported by MOST (973 Project: 2012CB82400). The work at the HFIR, ORNL, was sponsored by the Scientific User Facilities Division, BES, US DOE. NR 44 TC 14 Z9 14 U1 1 U2 26 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 17 PY 2013 VL 88 IS 13 AR 134512 DI 10.1103/PhysRevB.88.134512 PG 6 WC Physics, Condensed Matter SC Physics GA 240FY UT WOS:000326081600004 ER PT J AU Wu, DY Jospin, G Eisen, JA AF Wu, Dongying Jospin, Guillaume Eisen, Jonathan A. TI Systematic Identification of Gene Families for Use as "Markers" for Phylogenetic and Phylogeny-Driven Ecological Studies of Bacteria and Archaea and Their Major Subgroups SO PLOS ONE LA English DT Article ID RIBOSOMAL-RNA OPERON; SEQUENCE-ANALYSIS; GENOME; DATABASE; ALIGNMENTS; DIVERSITY; EVOLUTION; PROTEIN; TREES; INFERENCE AB With the astonishing rate that genomic and metagenomic sequence data sets are accumulating, there are many reasons to constrain the data analyses. One approach to such constrained analyses is to focus on select subsets of gene families that are particularly well suited for the tasks at hand. Such gene families have generally been referred to as "marker" genes. We are particularly interested in identifying and using such marker genes for phylogenetic and phylogeny-driven ecological studies of microbes and their communities (e. g., construction of species trees, phylogenetic based assignment of metagenomic sequence reads to taxonomic groups, phylogeny-based assessment of alpha-and beta-diversity of microbial communities from metagenomic data). We therefore refer to these as PhyEco (for phylogenetic and phylogenetic ecology) markers. The dual use of these PhyEco markers means that we needed to develop and apply a set of somewhat novel criteria for identification of the best candidates for such markers. The criteria we focused on included universality across the taxa of interest, ability to be used to produce robust phylogenetic trees that reflect as much as possible the evolution of the species from which the genes come, and low variation in copy number across taxa. We describe here an automated protocol for identifying potential PhyEco markers from a set of complete genome sequences. The protocol combines rapid searching, clustering and phylogenetic tree building algorithms to generate protein families that meet the criteria listed above. We report here the identification of PhyEco markers for different taxonomic levels including 40 for "all bacteria and archaea", 114 for "all bacteria (greatly expanding on the similar to 30 commonly used), and 100 s to 1000 s for some of the individual phyla of bacteria. This new list of PhyEco markers should allow much more detailed automated phylogenetic and phylogenetic ecology analyses of these groups than possible previously. C1 [Wu, Dongying; Jospin, Guillaume; Eisen, Jonathan A.] Univ Calif Davis, Genome Ctr, Dept Med Microbiol & Immunol, Dept Evolut & Ecol, Davis, CA 95616 USA. [Wu, Dongying] US DOE, Joint Genome Inst, Walnut Creek, CA USA. RP Wu, DY (reprint author), Univ Calif Davis, Genome Ctr, Dept Med Microbiol & Immunol, Dept Evolut & Ecol, Davis, CA 95616 USA. EM dygwu@ucdavis.edu OI Eisen, Jonathan A./0000-0002-0159-2197 FU Gordon and Betty Moore Foundation [1660, 3300] FX Funding for this work was provided by the Gordon and Betty Moore Foundation (grant #1660 and #3300, website: http://www.moore.org/). The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 54 TC 33 Z9 33 U1 1 U2 35 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD OCT 17 PY 2013 VL 8 IS 10 AR e77033 DI 10.1371/journal.pone.0077033 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 239KL UT WOS:000326022200029 PM 24146954 ER PT J AU Kasen, D AF Kasen, Daniel TI ASTROPHYSICS Super-luminous supernovae on the rise SO NATURE LA English DT Editorial Material ID PAIR-INSTABILITY; LIGHT CURVES; EXPLOSIONS; MAGNETAR; BIRTH C1 [Kasen, Daniel] Univ Calif Berkeley, Dept Phys & Astron, Berkeley, CA 94720 USA. [Kasen, Daniel] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. RP Kasen, D (reprint author), Univ Calif Berkeley, Dept Phys & Astron, Berkeley, CA 94720 USA. EM kasen@berkeley.edu NR 12 TC 1 Z9 1 U1 0 U2 4 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD OCT 17 PY 2013 VL 502 IS 7471 BP 310 EP 312 PG 3 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 235GY UT WOS:000325706300038 PM 24132286 ER PT J AU Lu, HY Schumacher, RA Adhikari, KP Adikaram, D Aghasyan, M Amaryan, MJ Pereira, SA Ball, J Battaglieri, M Batourine, V Bedlinskiy, I Biselli, AS Boiarinov, S Briscoe, WJ Brooks, WK Burkert, VD Carman, DS Celentano, A Chandavar, S Cole, PL Collins, P Contalbrigo, M Cortes, O Crede, V D'Angelo, A Dashyan, N De Vita, R De Sanctis, E Deur, A Djalali, C Doughty, D Dupre, R Egiyan, H El Alaoui, A El Fassi, L Eugenio, P Fedotov, G Fegan, S Fleming, JA Gabrielyan, M Gevorgyan, N Gilfoyle, GP Giovanetti, KL Girod, FX Goetz, JT Gohn, W Golovatch, E Gothe, RW Griffioen, KA Guidal, M Guo, L Hafidi, K Hakobyan, H Harrison, N Heddle, D Hicks, K Ho, D Holtrop, M Hyde, CE Ilieva, Y Ireland, DG Ishkhanov, BS Isupov, EL Jo, HS Joo, K Keller, D Khandaker, M Kim, W Klein, A Klein, FJ Koirala, S Kubarovsky, A Kubarovsky, V Kuleshov, SV Lewis, S Livingston, K MacGregor, IJD Martinez, D Mayer, M McKinnon, B Meyer, CA Mineeva, T Mirazita, M Mokeev, V Montgomery, RA Moriya, K Moutarde, H Munevar, E Camacho, CM Nadel-Turonski, P Nepali, CS Niccolai, S Niculescu, G Niculescu, I Osipenko, M Ostrovidov, AI Pappalardo, LL Paremuzyan, R Park, K Park, S Pasyuk, E Peng, P Phelps, E Phillips, JJ Pisano, S Pogorelko, O Pozdniakov, S Price, JW Procureur, S Prok, Y Protopopescu, D Puckett, AJR Raue, BA Rimal, D Ripani, M Rosner, G Rossi, P Sabatie, F Saini, MS Salgado, C Schott, D Seder, E Seraydaryan, H Sharabian, YG Smith, GD Sober, DI Sokhan, D Stepanyan, SS Stoler, P Strauch, S Taiuti, M Tang, W Tian, Y Tkachenko, S Torayev, B Vernarsky, B Voskanyan, H Voutier, E Walford, NK Weygand, DP Wood, MH Zachariou, N Zana, L Zhang, J Zhao, ZW AF Lu, H. Y. Schumacher, R. A. Adhikari, K. P. Adikaram, D. Aghasyan, M. Amaryan, M. J. Pereira, S. Anefalos Ball, J. Battaglieri, M. Batourine, V. Bedlinskiy, I. Biselli, A. S. Boiarinov, S. Briscoe, W. J. Brooks, W. K. Burkert, V. D. Carman, D. S. Celentano, A. Chandavar, S. Cole, P. L. Collins, P. Contalbrigo, M. Cortes, O. Crede, V. D'Angelo, A. Dashyan, N. De Vita, R. De Sanctis, E. Deur, A. Djalali, C. Doughty, D. Dupre, R. Egiyan, H. El Alaoui, A. El Fassi, L. Eugenio, P. Fedotov, G. Fegan, S. Fleming, J. A. Gabrielyan, M. Gevorgyan, N. Gilfoyle, G. P. Giovanetti, K. L. Girod, F. X. Goetz, J. T. Gohn, W. Golovatch, E. Gothe, R. W. Griffioen, K. A. Guidal, M. Guo, L. Hafidi, K. Hakobyan, H. Harrison, N. Heddle, D. Hicks, K. Ho, D. Holtrop, M. Hyde, C. E. Ilieva, Y. Ireland, D. G. Ishkhanov, B. S. Isupov, E. L. Jo, H. S. Joo, K. Keller, D. Khandaker, M. Kim, W. Klein, A. Klein, F. J. Koirala, S. Kubarovsky, A. Kubarovsky, V. Kuleshov, S. V. Lewis, S. Livingston, K. MacGregor, I. J. D. Martinez, D. Mayer, M. McKinnon, B. Meyer, C. A. Mineeva, T. Mirazita, M. Mokeev, V. Montgomery, R. A. Moriya, K. Moutarde, H. Munevar, E. Camacho, C. Munoz Nadel-Turonski, P. Nepali, C. S. Niccolai, S. Niculescu, G. Niculescu, I. Osipenko, M. Ostrovidov, A. I. Pappalardo, L. L. Paremuzyan, R. Park, K. Park, S. Pasyuk, E. Peng, P. Phelps, E. Phillips, J. J. Pisano, S. Pogorelko, O. Pozdniakov, S. Price, J. W. Procureur, S. Prok, Y. Protopopescu, D. Puckett, A. J. R. Raue, B. A. Rimal, D. Ripani, M. Rosner, G. Rossi, P. Sabatie, F. Saini, M. S. Salgado, C. Schott, D. Seder, E. Seraydaryan, H. Sharabian, Y. G. Smith, G. D. Sober, D. I. Sokhan, D. Stepanyan, S. S. Stoler, P. Strauch, S. Taiuti, M. Tang, W. Tian, Ye Tkachenko, S. Torayev, B. Vernarsky, B. Voskanyan, H. Voutier, E. Walford, N. K. Weygand, D. P. Wood, M. H. Zachariou, N. Zana, L. Zhang, J. Zhao, Z. W. CA CLAS Collaboration TI First observation of the Lambda(1405) line shape in electroproduction SO PHYSICAL REVIEW C LA English DT Article ID QUARK-MODEL; HYPERFINE INTERACTIONS; NUCLEON INTERACTIONS; CHIRAL DYNAMICS; BARYONS; SCATTERING; CONSTRAINTS; STATES AB We report the first observation of the line shape of the Lambda(1405) from electroproduction, and show that it is not a simple Breit-Wigner resonance. Electroproduction of K+ Lambda(1405) off the proton was studied by using data from CLAS at Jefferson Lab in the range 1.0 < Q(2) < 3.0 (GeV/c)(2). The analysis utilized the decay channels Sigma(+)pi(-) of the Lambda(1405) and p pi(0) of the Sigma(+). Neither the standard Particle Data Group resonance parameters, nor free parameters fitting to a single Breit-Wigner resonance represent the line shape. In our fits, the line shape corresponds approximately to predictions of a two-pole meson-baryon picture of the Lambda(1405), with a lower mass pole near 1368 MeV/c(2) and a higher mass pole near 1423 MeV/c(2). Furthermore, with increasing photon virtuality the mass distribution shifts toward the higher mass pole. C1 [Lu, H. Y.; Schumacher, R. A.; Biselli, A. S.; Ho, D.; Meyer, C. A.; Moriya, K.; Vernarsky, B.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [El Alaoui, A.; El Fassi, L.; Hafidi, K.] Argonne Natl Lab, Argonne, IL 60439 USA. [Pasyuk, E.] Arizona State Univ, Tempe, AZ 85287 USA. [Price, J. W.] Calif State Univ Dominguez Hills, Carson, CA 90747 USA. [Wood, M. H.] Canisius Coll, Buffalo, NY 14208 USA. [Collins, P.; Klein, F. J.; Sober, D. I.; Walford, N. K.] Catholic Univ Amer, Washington, DC 20064 USA. [Ball, J.; Moutarde, H.; Procureur, S.; Sabatie, F.] CEA, Ctr Saclay, Irfu Serv Phys Nucl, F-91191 Gif Sur Yvette, France. [Doughty, D.; Heddle, D.] Christopher Newport Univ, Newport News, VA 23606 USA. [Gohn, W.; Harrison, N.; Joo, K.; Kubarovsky, A.; Mineeva, T.; Seder, E.] Univ Connecticut, Storrs, CT 06269 USA. [Fleming, J. A.] Univ Edinburgh, Edinburgh EH9 3JZ, Midlothian, Scotland. [Biselli, A. S.] Fairfield Univ, Fairfield, CT 06824 USA. [Gabrielyan, M.; Guo, L.; Raue, B. A.; Rimal, D.] Florida Int Univ, Miami, FL 33199 USA. [Crede, V.; Eugenio, P.; Ostrovidov, A. I.; Park, S.; Saini, M. S.] Florida State Univ, Tallahassee, FL 32306 USA. [Taiuti, M.] Univ Genoa, I-16146 Genoa, Italy. [Briscoe, W. J.; Ilieva, Y.; Schott, D.; Strauch, S.] George Washington Univ, Washington, DC 20052 USA. [Cole, P. L.; Cortes, O.; Martinez, D.] Idaho State Univ, Pocatello, ID 83209 USA. [Contalbrigo, M.; Pappalardo, L. L.] Ist Nazl Fis Nucl, Sez Ferrara, I-44100 Ferrara, Italy. [Aghasyan, M.; Pereira, S. Anefalos; De Sanctis, E.; Mirazita, M.; Pisano, S.; Rossi, P.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Battaglieri, M.; Celentano, A.; De Vita, R.; Fegan, S.; Osipenko, M.; Ripani, M.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [D'Angelo, A.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, I-00133 Rome, Italy. [Dupre, R.; Guidal, M.; Jo, H. S.; Camacho, C. Munoz; Niccolai, S.; Paremuzyan, R.] Inst Phys Nucl ORSAY, Orsay, France. [Bedlinskiy, I.; Kuleshov, S. V.; Pogorelko, O.; Pozdniakov, S.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Giovanetti, K. L.; Niculescu, G.; Niculescu, I.] James Madison Univ, Harrisonburg, VA 22807 USA. [Kim, W.; Park, K.; Stepanyan, S. S.] Kyungpook Natl Univ, Taegu 702701, South Korea. [Voutier, E.] Univ Grenoble 1, CNRS, IN2P3, LPSC,INPG, Grenoble, France. [Holtrop, M.; Zana, L.] Univ New Hampshire, Durham, NH 03824 USA. [Khandaker, M.; Salgado, C.] Norfolk State Univ, Norfolk, VA 23504 USA. [Chandavar, S.; Goetz, J. T.; Hicks, K.; Niculescu, G.; Tang, W.] Ohio Univ, Athens, OH 45701 USA. [Adhikari, K. P.; Adikaram, D.; Amaryan, M. J.; Hyde, C. E.; Klein, A.; Koirala, S.; Mayer, M.; Nepali, C. S.; Prok, Y.; Seraydaryan, H.; Tkachenko, S.; Torayev, B.] Old Dominion Univ, Norfolk, VA 23529 USA. [Kubarovsky, V.; Stoler, P.] Rensselaer Polytech Inst, Troy, NY 12180 USA. [Gilfoyle, G. P.] Univ Richmond, Richmond, VA 23173 USA. [D'Angelo, A.] Univ Roma Tor Vergata, I-00133 Rome, Italy. [Fedotov, G.; Golovatch, E.; Ishkhanov, B. S.; Isupov, E. L.; Kubarovsky, A.; Mokeev, V.] Skobeltsyn Nucl Phys Inst, Moscow 119899, Russia. [Djalali, C.; Fedotov, G.; Gothe, R. W.; Ilieva, Y.; Phelps, E.; Strauch, S.; Tian, Ye; Wood, M. H.; Zachariou, N.] Univ S Carolina, Columbia, SC 29208 USA. [Batourine, V.; Boiarinov, S.; Brooks, W. K.; Burkert, V. D.; Carman, D. S.; Cole, P. L.; Deur, A.; Doughty, D.; Egiyan, H.; Girod, F. X.; Guo, L.; Heddle, D.; Kubarovsky, V.; Mokeev, V.; Munevar, E.; Nadel-Turonski, P.; Park, K.; Pasyuk, E.; Prok, Y.; Puckett, A. J. R.; Raue, B. A.; Sharabian, Y. G.; Weygand, D. P.; Zhang, J.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. [Brooks, W. K.; Hakobyan, H.; Kuleshov, S. V.] Univ Tecn Federico Santa Maria, Valparaiso, Chile. [Ireland, D. G.; Lewis, S.; Livingston, K.; MacGregor, I. J. D.; McKinnon, B.; Montgomery, R. A.; Phillips, J. J.; Protopopescu, D.; Rosner, G.; Smith, G. D.; Sokhan, D.] Univ Glasgow, Glasgow G12 8QQ, Lanark, Scotland. [Keller, D.; Peng, P.; Prok, Y.; Tkachenko, S.; Zhao, Z. W.] Univ Virginia, Charlottesville, VA 22901 USA. [Griffioen, K. A.] Coll William & Mary, Williamsburg, VA 23187 USA. [Dashyan, N.; Gevorgyan, N.; Hakobyan, H.; Voskanyan, H.] Yerevan Phys Inst, Yerevan 375036, Armenia. RP Lu, HY (reprint author), Univ Iowa, Iowa City, IA 52242 USA. EM schumacher@cmu.edu RI Adikaram, D/H-7128-2016; Celentano, Andrea/J-6190-2012; Lu, Haiyun/B-4083-2012; Ireland, David/E-8618-2010; El Alaoui, Ahmed/B-4638-2015; Brooks, William/C-8636-2013; Ishkhanov, Boris/E-1431-2012; Schumacher, Reinhard/K-6455-2013; Sabatie, Franck/K-9066-2015; Osipenko, Mikhail/N-8292-2015; MacGregor, Ian/D-4072-2011; D'Angelo, Annalisa/A-2439-2012; Meyer, Curtis/L-3488-2014; Zhang, Jixie/A-1461-2016; Adikaram, Dasuni/D-1539-2016 OI Celentano, Andrea/0000-0002-7104-2983; Ireland, David/0000-0001-7713-7011; Brooks, William/0000-0001-6161-3570; Schumacher, Reinhard/0000-0002-3860-1827; Sabatie, Franck/0000-0001-7031-3975; Osipenko, Mikhail/0000-0001-9618-3013; D'Angelo, Annalisa/0000-0003-3050-4907; Meyer, Curtis/0000-0001-7599-3973; FU DOE [DE-FG02-87ER40315]; United States Department of Energy [DE-AC05-84ER40150]; National Science Foundation; United Kingdom's Science and Technology Facilities Council (STFC); National Research Foundation of Korea FX We acknowledge the outstanding efforts of the staff of the Accelerator and Physics Divisions at Jefferson Lab that made this experiment possible. The work of the Medium Energy Physics group at Carnegie Mellon University was supported by DOE Grant No. DE-FG02-87ER40315. The Southeastern Universities Research Association (SURA) operated the Thomas Jefferson National Accelerator Facility for the United States Department of Energy under Contract No. DE-AC05-84ER40150. Support was also provided by the National Science Foundation, the United Kingdom's Science and Technology Facilities Council (STFC), and the National Research Foundation of Korea. NR 29 TC 9 Z9 9 U1 0 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD OCT 17 PY 2013 VL 88 IS 4 AR 045202 DI 10.1103/PhysRevC.88.045202 PG 7 WC Physics, Nuclear SC Physics GA 240KV UT WOS:000326095700003 ER PT J AU Wu, D Dong, XQ Xi, BK Feng, Z Kennedy, A Mullendore, G Gilmore, M Tao, WK AF Wu, Di Dong, Xiquan Xi, Baike Feng, Zhe Kennedy, Aaron Mullendore, Gretchen Gilmore, Matthew Tao, Wei-Kuo TI Impacts of microphysical scheme on convective and stratiform characteristics in two high precipitation squall line events SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article ID CLOUD-RESOLVING MODEL; NUMERICAL SIMULATIONS; PART I; BULK PARAMETERIZATION; TROPICAL CONVECTION; ISOLATED MICROBURST; SENSITIVITY; ICE; MESOSCALE; DYNAMICS C1 [Wu, Di; Dong, Xiquan; Xi, Baike; Feng, Zhe; Kennedy, Aaron; Mullendore, Gretchen; Gilmore, Matthew] Univ N Dakota, Dept Atmospher Sci, Grand Forks, ND 58202 USA. [Wu, Di; Tao, Wei-Kuo] NASA Goddard Space Flight Ctr, Greenbelt, MD USA. [Feng, Zhe] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Dong, XQ (reprint author), Univ N Dakota, Dept Atmospher Sci, 4149 Univ Ave,Stop 9006, Grand Forks, ND 58202 USA. EM dong@aero.und.edu RI Feng, Zhe/D-9531-2013; Feng, Zhe/E-1877-2015; OI Feng, Zhe/0000-0002-7540-9017; Dong, Xiquan/0000-0002-3359-6117 FU U.S. Department of Energy Office of Energy Research, Office of Health and Environmental Research, Environmental Sciences Division; NOAA GOES-R project [NA11NES440004]; DOE ASR project [DE-SC0008468]; NASA EPSCoR CAN [NNX11AM15A]; DOE Atmospheric System Research (ASR) program FX Surface data and Oklahoma Mesonet precipitation were obtained from the Atmospheric Radiation Measurement Program sponsored by the U.S. Department of Energy Office of Energy Research, Office of Health and Environmental Research, Environmental Sciences Division. We are in debt to Song-You Hong from Yonsei University for providing reflectivity calculation algorithm based on WSM6 scheme. Comments from three anonymous reviewers improved the manuscript and are appreciated. We are also very grateful to Samson Hagos at PNNL for his constructive comments. This research was primarily supported by NOAA GOES-R project managed by Ingrid Guch and Mark DeMaria with award NA11NES440004 at the University of North Dakota. The University of North Dakota authors were also supported by DOE ASR project with award number DE-SC0008468, and NASA EPSCoR CAN under grant NNX11AM15A. The PNNL author is also supported by the DOE Atmospheric System Research (ASR) program. NR 50 TC 13 Z9 13 U1 1 U2 14 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD OCT 16 PY 2013 VL 118 IS 19 BP 11119 EP 11135 DI 10.1002/jgrd.50798 PG 17 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 297PF UT WOS:000330266700044 ER PT J AU Olaguer, EP Herndon, SC Buzcu-Guven, B Kolb, CE Brown, MJ Cuclis, AE AF Olaguer, Eduardo P. Herndon, Scott C. Buzcu-Guven, Birnur Kolb, Charles E. Brown, Michael J. Cuclis, Alex E. TI Attribution of primary formaldehyde and sulfur dioxide at Texas City during SHARP/formaldehyde and olefins from large industrial releases (FLAIR) using an adjoint chemistry transport model SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article ID URBAN; DISTRIBUTIONS; FLARES C1 [Olaguer, Eduardo P.; Buzcu-Guven, Birnur; Cuclis, Alex E.] Houston Adv Res Ctr, The Woodlands, TX 77381 USA. [Herndon, Scott C.; Kolb, Charles E.] Aerodyne Res Inc, Billerica, MA USA. [Brown, Michael J.] Los Alamos Natl Lab, Los Alamos, NM USA. RP Olaguer, EP (reprint author), Houston Adv Res Ctr, 4800 Res Forest Dr, The Woodlands, TX 77381 USA. EM eolaguer@harc.edu RI Kolb, Charles/A-8596-2009 FU U.S. Department of the Interior, Fish and Wildlife Service, Coastal Impact Assistance Program through Harris County, Texas FX We would like to acknowledge Bernhard Rappengluck for providing access to the University of Houston's Piper Aztec data set for the FLAIR campaign and Jochen Stutz of the University of California at Los Angeles for his helpful comments and suggestions. This work was supported by the U.S. Department of the Interior, Fish and Wildlife Service, Coastal Impact Assistance Program through Harris County, Texas. NR 19 TC 7 Z9 7 U1 0 U2 8 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD OCT 16 PY 2013 VL 118 IS 19 BP 11317 EP 11326 DI 10.1002/jgrd.50794 PG 10 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 297PF UT WOS:000330266700046 ER PT J AU Jeong, S Hsu, YK Andrews, AE Bianco, L Vaca, P Wilczak, JM Fischer, ML AF Jeong, Seongeun Hsu, Ying-Kuang Andrews, Arlyn E. Bianco, Laura Vaca, Patrick Wilczak, James M. Fischer, Marc L. TI A multitower measurement network estimate of California's methane emissions SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article ID CONVECTIVE BOUNDARY-LAYER; LOS-ANGELES BASIN; CARBON-DIOXIDE; STILT MODEL; DEPTH; INDEX C1 [Jeong, Seongeun; Fischer, Marc L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Hsu, Ying-Kuang; Vaca, Patrick] Calif Air Resources Board, Sacramento, CA USA. [Andrews, Arlyn E.; Bianco, Laura; Wilczak, James M.] NOAA, Earth Syst Res Lab, Boulder, CO USA. [Bianco, Laura] Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA. [Fischer, Marc L.] Calif State Univ East Bay, Dept Anthropol Geog & Environm Studies, Hayward, CA USA. RP Jeong, S (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, MS 90R2002,1 Cyclotron Rd, Berkeley, CA 94720 USA. EM sjeong@lbl.gov RI Andrews, Arlyn/K-3427-2012 FU CARB [09-348]; U.S. Department of Energy [DE-AC02-05CH11231]; NOAA USWRP; HOA; Atmospheric Composition and Climate Program; Carbon Cycle Program of NOAA's Climate Program Office FX We thank Dave Field, Dave Bush, Edward Wahl, Ken Reichl, Fabien Guerin, Yuchen Yi, and particularly Jon Kofler for assistance with measurements at WGC and analysis of data from radar wind profiler sites, John Lin, Christoph Gerbig, Steve Wofsy, Janusz Eluszkiewicz, Thomas Nehrkorn for sharing the STILT code and advice, Chris Potter and William Salas for sharing modeled CH4 emission for use as a priori estimates, Ed Dlugokencky and Colm Sweeney for sharing data for CH4 background estimates, Larry Hunsaker, Marc Vayssieres, Joseph Fischer, and Webster Tassat for sharing CARB CH4 emissions information, and Krishna Muriki for assistance running the WRF-STILT models on the LBNL-Lawrencium cluster. We thank Ken Davis and two anonymous reviewers for providing thoughtful comments and suggestions. We also thank Guido Franco, Jorn Horner, and Eileen McCauley for useful advice, and David Larson for institutional support at CSU East Bay. This analysis was supported by CARB (contract 09-348), data collection at Walnut Grove by the California Energy Commissions Public Interest Environmental Research program, with work at LBNL conducted under U.S. Department of Energy contract DE-AC02-05CH11231. Support for L. Bianco and J. Wilczak was provided by NOAA USWRP and HOA program funding. NOAA measurements were funded in part by the Atmospheric Composition and Climate Program and the Carbon Cycle Program of NOAA's Climate Program Office. NR 39 TC 29 Z9 30 U1 0 U2 7 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD OCT 16 PY 2013 VL 118 IS 19 BP 11339 EP 11351 DI 10.1002/jgrd.50854 PG 13 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 297PF UT WOS:000330266700031 ER PT J AU Ashfaq, M Ghosh, S Kao, SC Bowling, LC Mote, P Touma, D Rauscher, SA Diffenbaugh, NS AF Ashfaq, Moetasim Ghosh, Subimal Kao, Shih-Chieh Bowling, Laura C. Mote, Philip Touma, Danielle Rauscher, Sara A. Diffenbaugh, Noah S. TI Near-term acceleration of hydroclimatic change in the western US SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article ID CLIMATE-CHANGE COMMITMENT; COLORADO RIVER-BASIN; CHANGE-TYPE DROUGHT; UNITED-STATES; WATER-RESOURCES; SNOWMELT RUNOFF; NORTH-AMERICA; MOUNTAIN SNOWPACK; CHANGE SCENARIOS; DIE-OFF C1 [Ashfaq, Moetasim; Kao, Shih-Chieh; Touma, Danielle] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Ashfaq, Moetasim; Diffenbaugh, Noah S.] Stanford Univ, Woods Inst Environm, Stanford, CA 94305 USA. [Ashfaq, Moetasim; Diffenbaugh, Noah S.] Stanford Univ, Dept Environm Earth Syst Sci, Stanford, CA 94305 USA. [Ashfaq, Moetasim; Bowling, Laura C.; Diffenbaugh, Noah S.] Purdue Univ, Purdue Climate Change Res Ctr, W Lafayette, IN 47907 USA. [Ashfaq, Moetasim; Diffenbaugh, Noah S.] Purdue Univ, Dept Earth Atmospher & Planetary Sci, W Lafayette, IN 47907 USA. [Ghosh, Subimal] Indian Inst Technol, Dept Civil Engn, Bombay 400076, Maharashtra, India. [Bowling, Laura C.] Purdue Univ, Dept Agron, W Lafayette, IN 47907 USA. [Mote, Philip] Oregon State Univ, Oregon Climate Change Res Inst, Corvallis, OR 97331 USA. [Mote, Philip] Oregon State Univ, Oregon Climate Serv, Corvallis, OR 97331 USA. [Rauscher, Sara A.] Univ Delaware, Dept Geog, Newark, DE USA. RP Ashfaq, M (reprint author), Oak Ridge Natl Lab, POB MS6301, Oak Ridge, TN 37831 USA. EM mashfaq@ornl.gov RI Diffenbaugh, Noah/I-5920-2014; Kao, Shih-Chieh/B-9428-2012; Bowling, Laura/B-6963-2013; OI Diffenbaugh, Noah/0000-0002-8856-4964; Kao, Shih-Chieh/0000-0002-3207-5328; Bowling, Laura/0000-0002-1439-3154; Touma, Danielle/0000-0003-1992-9904; Ghosh, Subimal/0000-0002-5722-1440 FU NSF [0955283]; DOE [3ERKP777, DE-FG02-08ER64649, DE-SC0001483]; ORNL LDRD [32112413] FX We thank two editors and five anonymous reviewers for their insightful and constructive comments through five submissions over the past two years. We thank the Rosen Center for Advanced Computing (RCAC) at Purdue University for access to computing resources. We thank the modeling groups, the WCRP's WGCM, PCMDI, and the U.S. DOE for enabling the CMIP3 and CMIP5 archives, the North American Regional Climate Change Assessment Program for the NARCCAP archive, the Oregon State University for PRISM data, and the USGS for WaterWatch data. This work was supported by NSF award 0955283; DOE awards 3ERKP777, DE-FG02-08ER64649, and DE-SC0001483; and ORNL LDRD award 32112413. NR 98 TC 23 Z9 23 U1 7 U2 39 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD OCT 16 PY 2013 VL 118 IS 19 BP 10676 EP 10693 DI 10.1002/jgrd.50816 PG 18 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 297PF UT WOS:000330266700016 ER PT J AU Tilmes, S Fasullo, J Lamarque, JF Marsh, DR Mills, M Alterskjaer, K Muri, H Kristjansson, JE Boucher, O Schulz, M Cole, JNS Curry, CL Jones, A Haywood, J Irvine, PJ Ji, DY Moore, JC Karam, DB Kravitz, B Rasch, PJ Singh, B Yoon, JH Niemeier, U Schmidt, H Robock, A Yang, ST Watanabe, S AF Tilmes, Simone Fasullo, John Lamarque, Jean-Francois Marsh, Daniel R. Mills, Michael Alterskjaer, Kari Muri, Helene Kristjansson, Jon E. Boucher, Olivier Schulz, Michael Cole, Jason N. S. Curry, Charles L. Jones, Andy Haywood, Jim Irvine, Peter J. Ji, Duoying Moore, John C. Karam, Diana B. Kravitz, Ben Rasch, Philip J. Singh, Balwinder Yoon, Jin-Ho Niemeier, Ulrike Schmidt, Hauke Robock, Alan Yang, Shuting Watanabe, Shingo TI The hydrological impact of geoengineering in the Geoengineering Model Intercomparison Project (GeoMIP) SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article ID COMMUNITY ATMOSPHERE MODEL; EARTHS RADIATION BALANCE; LARGE-SCALE MODELS; CLIMATE-CHANGE; OZONE DEPLETION; MOUNT-PINATUBO; CUMULUS PARAMETERIZATION; GLOBAL PRECIPITATION; CLOUD ENSEMBLE; CYCLE C1 [Tilmes, Simone; Fasullo, John; Lamarque, Jean-Francois; Marsh, Daniel R.; Mills, Michael] Natl Ctr Atmospher Res, Boulder, CO 80305 USA. [Alterskjaer, Kari; Muri, Helene; Kristjansson, Jon E.] Univ Oslo, Dept Geosci, Meteorol & Oceanog Sect, Oslo, Norway. [Boucher, Olivier; Schulz, Michael] CNRS UPMC, Lab Meteorol Dynam, IPSL, Paris, France. [Cole, Jason N. S.] Environm Canada, Canadian Ctr Climate Modeling & Anal, Toronto, ON, Canada. [Curry, Charles L.] Univ Victoria, Sch Earth & Ocean Sci, Victoria, BC, Canada. [Jones, Andy; Haywood, Jim] Met Off Hadley Ctr, Exeter, Devon, England. [Haywood, Jim] Univ Exeter, Exeter Climate Syst, Exeter, Devon, England. [Irvine, Peter J.] Inst Adv Sustainabil Studies, Potsdam, Germany. [Ji, Duoying; Moore, John C.] Beijing Normal Univ, State Key Lab Earth Surface Proc & Resource Ecol, Coll Global Change & Earth Syst Sci, Beijing 100875, Peoples R China. [Karam, Diana B.] UVSQ, CNRS, Lab Sci Climat & Environm, CEA, Gif Sur Yvette, France. [Kravitz, Ben; Rasch, Philip J.; Singh, Balwinder; Yoon, Jin-Ho] Pacific NW Natl Lab, Richland, WA 99352 USA. [Niemeier, Ulrike; Schmidt, Hauke] Max Planck Inst Meteorol, D-20146 Hamburg, Germany. [Robock, Alan] Rutgers State Univ, Dept Environm Sci, New Brunswick, NJ 08903 USA. [Yang, Shuting] Danish Meteorol Inst, Copenhagen, Denmark. [Watanabe, Shingo] Japan Agcy Marine Earth Sci & Technol, Yokohama, Kanagawa, Japan. RP Tilmes, S (reprint author), Natl Ctr Atmospher Res, 1850 Table Mesa Dr,3450 Mitchell Lane, Boulder, CO 80305 USA. EM tilmes@ucar.edu RI Moore, John/B-2868-2013; YOON, JIN-HO/A-1672-2009; Marsh, Daniel/A-8406-2008; Lamarque, Jean-Francois/L-2313-2014; Kravitz, Ben/P-7925-2014; Muri, Helene/D-4845-2015; Schulz, Michael/A-6930-2011; Robock, Alan/B-6385-2016; Mills, Michael/B-5068-2010; Watanabe, Shingo/L-9689-2014 OI Cole, Jason/0000-0003-0450-2748; Moore, John/0000-0001-8271-5787; YOON, JIN-HO/0000-0002-4939-8078; Marsh, Daniel/0000-0001-6699-494X; Lamarque, Jean-Francois/0000-0002-4225-5074; Kravitz, Ben/0000-0001-6318-1150; Muri, Helene/0000-0003-4738-493X; Schulz, Michael/0000-0003-4493-4158; Mills, Michael/0000-0002-8054-1346; Watanabe, Shingo/0000-0002-2228-0088 FU NASA [NNG06GB91G]; DECC/Defra Met Office Hadley Centre Climate Programme [GA01101]; European Unions [226567-IMPLICC]; Fund for Innovative Climate and Energy Research; NASA High-End Computing (HEC) Program through the NASA Center for Climate Simulation (NCCS) at Goddard Space Flight Center; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; NERSC; EU [306395]; U.S. National Science Foundation [AGS-1157525]; SOUSEI Program, MEXT, Japan; National Science Foundation FX We thank all participants of the Geoengineering Model Intercomparison Project and their model development teams, the CLIVAR/WCRP Working Group on Coupled Modeling for endorsing GeoMIP, and the scientists managing the Earth System Grid data nodes who have assisted with making GeoMIP output available. We further acknowledge the World Climate Research Programme's Working Group on Coupled Modelling, which is responsible for CMIP, and we thank the climate modeling groups for producing and making available their model output. For CMIP, the U.S. Department of Energy's Program for Climate Model Diagnosis and Intercomparison provides coordinating support and led development of software infrastructure in partnership with the Global Organization for Earth System Science Portals. We thank the TRMM Online Visualization and Analysis System (TOVAS) and the GPCC Global Precipitation Climatology Centre for providing the rainfall data set. The participation of J. Fasullo is supported by NASA Award NNG06GB91G. J. Haywood and A. Jones were supported by the joint DECC/Defra Met Office Hadley Centre Climate Programme (GA01101). K. Alterskjaer, D. B. Karam, J. E. Kristjansson, U. Niemeier, H. Schmidt, and M. Schulz received funding from the European Unions Seventh Framework Programme (FP7/2007-2013) under grant agreement 226567-IMPLICC. K. Alterskjaer and J.E. Kristjansson received support from the Norwegian Research Council's Programme for Supercomputing (NOTUR) through a grant of computing time. B. Kravitz is supported by the Fund for Innovative Climate and Energy Research. Simulations performed by B. Kravitz were supported by the NASA High-End Computing (HEC) Program through the NASA Center for Climate Simulation (NCCS) at Goddard Space Flight Center. Computer resources for P.J. Rasch, B. Singh, and J.-H. Yoon were provided by the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract DE-AC02-05CH11231. J.-H. Yoon was further supported by the NERSC. D. Ji and J. Moore thank all members of the BNU-ESM model group, as well as the Center of Information and Network Technology at Beijing Normal University for assistance in publishing the GeoMIP data set. H. Muri was supported by the EU 7th Framework Programme grant agreement 306395, EuTRACE. A. Robock is supported by the U.S. National Science Foundation grant AGS-1157525. S. Watanabe was supported by SOUSEI Program, MEXT, Japan, and the Earth Simulator was used for the simulations of MIROC-ESM. Finally, we thank Gary Strand for CCSM4 output formatting and James Hurrell for supporting this study. The National Center for Atmospheric Research is funded by the National Science Foundation. We thank all reviewers and Govindasamy Bala for useful suggestions to the paper. NR 81 TC 58 Z9 58 U1 6 U2 42 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD OCT 16 PY 2013 VL 118 IS 19 BP 11036 EP 11058 DI 10.1002/jgrd.50868 PG 23 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 297PF UT WOS:000330266700026 ER PT J AU Xu, YY Bahadur, R Zhao, C Leung, LR AF Xu, Yangyang Bahadur, Ranjit Zhao, Chun Leung, L. Ruby TI Estimating the radiative forcing of carbonaceous aerosols over California based on satellite and ground observations SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article ID BLACK CARBON; LIGHT-ABSORPTION; BROWN CARBON; OPTICAL-PROPERTIES; EMISSION FACTORS; ORGANIC-CARBON; CLIMATE; CLOUDS; MODEL; PARTICLES C1 [Xu, Yangyang; Bahadur, Ranjit] Univ Calif San Diego, Scripps Inst Oceanog, La Jolla, CA 92013 USA. [Zhao, Chun; Leung, L. Ruby] Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. RP Xu, YY (reprint author), Univ Calif San Diego, Scripps Inst Oceanog, La Jolla, CA 92013 USA. EM yangyang@ucsd.edu RI Zhao, Chun/A-2581-2012 OI Zhao, Chun/0000-0003-4693-7213 FU California Air Resources Board (CARB) [08-323]; National Science Foundation (NSF) [ATM 0721142]; Office of Science of the U.S. Department of Energy as part of the Regional and Global Climate Modeling program; DOE by Battelle Memorial Institute [DE-AC05-76RL01830] FX This work was supported by California Air Resources Board (CARB) under contract 08-323, National Science Foundation (NSF) under award ATM 0721142, and by the Office of Science of the U.S. Department of Energy as part of the Regional and Global Climate Modeling program. The Pacific Northwest National Laboratory is operated for DOE by Battelle Memorial Institute under contract DE-AC05-76RL01830. We acknowledge Prof. V. Ramanathan for his valuable comments on the work. We also thank D. Kim, P. S. Praveen, T. Ahmed, B. Chen, J. Burney, and D. Biasca for their help during various stages of this project. The NASA AERONET group and GES DISC Giovanni system provided some data sets used in this study. We are grateful to four anonymous reviewers for their valuable comments that greatly improved the presentation of the work. NR 64 TC 11 Z9 11 U1 2 U2 10 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD OCT 16 PY 2013 VL 118 IS 19 BP 11148 EP 11160 DI 10.1002/jgrd.50835 PG 13 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 297PF UT WOS:000330266700039 ER PT J AU Kravitz, B Forster, PM Jones, A Robock, A Alterskjaer, K Boucher, O Jenkins, AKL Korhonen, H Kristjansson, JE Muri, H Niemeier, U Partanen, AI Rasch, PJ Wang, HL Watanabe, S AF Kravitz, Ben Forster, Piers M. Jones, Andy Robock, Alan Alterskjaer, Kari Boucher, Olivier Jenkins, Annabel K. L. Korhonen, Hannele Kristjansson, Jon Egill Muri, Helene Niemeier, Ulrike Partanen, Antti-Ilari Rasch, Philip J. Wang, Hailong Watanabe, Shingo TI Sea spray geoengineering experiments in the geoengineering model intercomparison project (GeoMIP): Experimental design and preliminary results SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article ID MESOSCALE CELLULAR STRUCTURES; LEVEL MARITIME CLOUDS; EARTH-SYSTEM MODEL; ALBEDO ENHANCEMENT; MARINE; MICROPHYSICS; POLLUTION; IMPACT; STABILIZATION; PRECIPITATION C1 [Kravitz, Ben; Rasch, Philip J.; Wang, Hailong] Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. [Forster, Piers M.; Jenkins, Annabel K. L.] Univ Leeds, Sch Earth & Environm, Leeds, W Yorkshire, England. [Jones, Andy] Met Off Hadley Ctr, Exeter, Devon, England. [Robock, Alan] Rutgers State Univ, Dept Environm Sci, New Brunswick, NJ 08903 USA. [Alterskjaer, Kari; Kristjansson, Jon Egill; Muri, Helene] Univ Oslo, Dept Geosci, Oslo, Norway. [Boucher, Olivier] CNRS UPMC, Lab Meteorol Dynam, IPSL, Paris, France. [Korhonen, Hannele; Partanen, Antti-Ilari] Finnish Meteorol Inst, Kuopio Unit, Kuopio, Finland. [Niemeier, Ulrike] Max Planck Inst Meteorol, D-20146 Hamburg, Germany. [Watanabe, Shingo] Japan Agcy Marine Earth Sci & Technol, Yokohama, Kanagawa, Japan. RP Kravitz, B (reprint author), Pacific NW Natl Lab, Atmospher Sci & Global Change Div, POB 999,MSIN K9-24, Richland, WA 99352 USA. EM ben.kravitz@pnnl.gov RI Korhonen, Hannele/E-4489-2011; Wang, Hailong/B-8061-2010; Kravitz, Ben/P-7925-2014; Muri, Helene/D-4845-2015; Robock, Alan/B-6385-2016; Forster, Piers/F-9829-2010; Watanabe, Shingo/L-9689-2014; OI Korhonen, Hannele/0000-0001-6264-0706; Wang, Hailong/0000-0002-1994-4402; Kravitz, Ben/0000-0001-6318-1150; Muri, Helene/0000-0003-4738-493X; Forster, Piers/0000-0002-6078-0171; Watanabe, Shingo/0000-0002-2228-0088; Partanen, Antti-Ilari/0000-0002-0883-8161 FU Fund for Innovative Climate and Energy Research (FICER); U.S. Department of Energy by Battelle Memorial Institute [DE-AC05-76RL01830]; NASA High-End Computing (HEC) Program through the NASA Center for Climate Simulation (NCCS) at Goddard Space Flight Center; IAGP: EPSRC [EP/I014721/1]; Joint DECC/Defra Met Office Hadley Centre Climate Programme [GA01101]; NSF [AGS-1157525, CBET-1240507]; European Commission [FP7-ENV-2008-1-226567]; Norwegian Research Council through the EarthClim project and its program for supercomputing (NOTUR) [207711/E10]; EU [306395]; SOUSEI program, MEXT, Japan FX We thank the participants of the GeoMIP 2013 workshop, held at the Institute for Advanced Sustainability Studies in Potsdam, Germany on 15-16 April 2013 for helpful discussions regarding the experiment design, as well as two anonymous reviewers for their comments on this manuscript. Ben Kravitz is supported by the Fund for Innovative Climate and Energy Research (FICER). The Pacific Northwest National Laboratory is operated for the U.S. Department of Energy by Battelle Memorial Institute under contract DE-AC05-76RL01830. Simulations performed by Ben Kravitz were supported by the NASA High-End Computing (HEC) Program through the NASA Center for Climate Simulation (NCCS) at Goddard Space Flight Center. Piers M. Forster is supported by IAGP: EPSRC grant EP/I014721/1. Andy Jones is supported by the Joint DECC/Defra Met Office Hadley Centre Climate Programme (GA01101). Alan Robock is supported by NSF grants AGS-1157525 and CBET-1240507. Kari Alterskjaer was supported by the European Commission's 7th Framework Program through the IMPLICC project (FP7-ENV-2008-1-226567) and by the Norwegian Research Council through the EarthClim project (207711/E10) and its program for supercomputing (NOTUR) through a grant for computing time. Helene Muri is supported by the EU 7th Framework Programme under grant agreement 306395, EuTRACE. Shingo Watanabe is supported by the SOUSEI program, MEXT, Japan. NR 52 TC 10 Z9 11 U1 2 U2 16 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD OCT 16 PY 2013 VL 118 IS 19 BP 11175 EP 11186 DI 10.1002/jgrd.50856 PG 12 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 297PF UT WOS:000330266700028 ER PT J AU Shakya, M Gottel, N Castro, H Yang, ZMK Gunter, L Labbe, J Muchero, W Bonito, G Vilgalys, R Tuskan, G Podar, M Schadt, CW AF Shakya, Migun Gottel, Neil Castro, Hector Yang, Zamin K. Gunter, Lee Labbe, Jessy Muchero, Wellington Bonito, Gregory Vilgalys, Rytas Tuskan, Gerald Podar, Mircea Schadt, Christopher W. TI A Multifactor Analysis of Fungal and Bacterial Community Structure in the Root Microbiome of Mature Populus deltoides Trees SO PLOS ONE LA English DT Article ID MYCORRHIZAL FUNGI; BLACK COTTONWOOD; ECOLOGICAL DATA; RHIZOSPHERE; DIVERSITY; POPLAR; ENDOPHYTES; PLANTS; GROWTH; COEXISTENCE AB Bacterial and fungal communities associated with plant roots are central to the host health, survival and growth. However, a robust understanding of the root-microbiome and the factors that drive host associated microbial community structure have remained elusive, especially in mature perennial plants from natural settings. Here, we investigated relationships of bacterial and fungal communities in the rhizosphere and root endosphere of the riparian tree species Populus deltoides, and the influence of soil parameters, environmental properties (host phenotype and aboveground environmental settings), host plant genotype (Simple Sequence Repeat (SSR) markers), season (Spring vs. Fall) and geographic setting (at scales from regional watersheds to local riparian zones) on microbial community structure. Each of the trees sampled displayed unique aspects to its associated community structure with high numbers of Operational Taxonomic Units (OTUs) specific to an individual trees (bacteria >90%, fungi >60%). Over the diverse conditions surveyed only a small number of OTUs were common to all samples within rhizosphere (35 bacterial and 4 fungal) and endosphere (1 bacterial and 1 fungal) microbiomes. As expected, Proteobacteria and Ascomycota were dominant in root communities (>50%) while other higher-level phylogenetic groups (Chytridiomycota, Acidobacteria) displayed greatly reduced abundance in endosphere compared to the rhizosphere. Variance partitioning partially explained differences in microbiome composition between all sampled roots on the basis of seasonal and soil properties (4% to 23%). While most variation remains unattributed, we observed significant differences in the microbiota between watersheds (Tennessee vs. North Carolina) and seasons (Spring vs. Fall). SSR markers clearly delineated two host populations associated with the samples taken in TN vs. NC, but overall host genotypic distances did not have a significant effect on corresponding communities that could be separated from other measured effects. C1 [Shakya, Migun; Gottel, Neil; Castro, Hector; Yang, Zamin K.; Gunter, Lee; Labbe, Jessy; Muchero, Wellington; Tuskan, Gerald; Podar, Mircea; Schadt, Christopher W.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. [Shakya, Migun; Podar, Mircea; Schadt, Christopher W.] Univ Tennessee, Genome Sci & Technol Program, Knoxville, TN USA. [Castro, Hector; Podar, Mircea; Schadt, Christopher W.] Univ Tennessee, Dept Microbiol, Knoxville, TN 37996 USA. [Bonito, Gregory; Vilgalys, Rytas] Duke Univ, Dept Biol, Durham, NC USA. RP Schadt, CW (reprint author), Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. EM schadtcw@ornl.gov RI Schadt, Christopher/B-7143-2008; Gunter, Lee/L-3480-2016; Tuskan, Gerald/A-6225-2011; Labbe, Jessy/G-9532-2011; OI Schadt, Christopher/0000-0001-8759-2448; Gunter, Lee/0000-0003-1211-7532; Tuskan, Gerald/0000-0003-0106-1289; Labbe, Jessy/0000-0003-0368-2054; Podar, Mircea/0000-0003-2776-0205; Vilgalys, Rytas/0000-0001-8299-3605; muchero, wellington/0000-0002-0200-9856 FU Genomic Science Program, U.S. Department of Energy, Office of Science, Biological and Environmental Research, as part of the Plant Microbe Interfaces Scientific Focus Area; U.S. Department of Energy [DE-AC05-00OR22725] FX This research was sponsored by the Genomic Science Program, U.S. Department of Energy, Office of Science, Biological and Environmental Research, as part of the Plant Microbe Interfaces Scientific Focus Area (http://pmi.ornl.gov). Oak Ridge National Laboratory is managed by UT-Battelle LLC, for the U.S. Department of Energy under contract DE-AC05-00OR22725. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 63 TC 46 Z9 47 U1 14 U2 137 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD OCT 16 PY 2013 VL 8 IS 10 AR e76382 DI 10.1371/journal.pone.0076382 PG 12 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 239JR UT WOS:000326019400057 PM 24146861 ER PT J AU Magazu, S Frauenfelder, H AF Magazu, Salvatore Frauenfelder, Hans TI Editorial of Special Issue of Chemical Physics "Neutrons Scattering Highlights on Water and Biological Systems" SO CHEMICAL PHYSICS LA English DT Editorial Material C1 [Magazu, Salvatore] Univ Messina, Dipartimento Fis & Sci Terra, I-98166 Messina, Italy. [Frauenfelder, Hans] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Magazu, S (reprint author), Univ Messina, Dipartimento Fis & Sci Terra, Viale Ferdinando Stagno DAlcontres 31,POB 55, I-98166 Messina, Italy. EM smagazu@unime.it; hansfrauenfelder@me.com NR 0 TC 0 Z9 0 U1 1 U2 4 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0301-0104 EI 1873-4421 J9 CHEM PHYS JI Chem. Phys. PD OCT 16 PY 2013 VL 424 BP 1 EP 1 DI 10.1016/j.chemphys.2013.09.009 PG 1 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 252DA UT WOS:000326983700001 ER PT J AU Fenimore, PW Frauenfelder, H Magazu, S McMahon, BH Mezei, F Migliardo, F Young, RD Stroe, I AF Fenimore, Paul W. Frauenfelder, Hans Magazu, Salvatore McMahon, Benjamin H. Mezei, Ferenc Migliardo, Federica Young, Robert D. Stroe, Izabela TI Concepts and problems in protein dynamics SO CHEMICAL PHYSICS LA English DT Article DE Protein dynamics; Neutron scattering; Mossbauer spectroscopy ID MEAN-SQUARE DISPLACEMENTS; X-RAY-DIFFRACTION; RESONANCE ABSORPTION; HYDRATED MYOGLOBIN; ENERGY LANDSCAPES; GAMMA-RAYS; TRANSITION; SOLVENT; FLUCTUATIONS; MOSSBAUER AB The function of proteins depends crucially on conformational motions. The characteristic times of these motions extend from sub-picosecond to seconds. No single experimental tool can cover the entire time range and provide all necessary parameters for a complete understanding. Moreover, without a solid understanding of the data evaluation it is easy to misinterpret the complex phenomena. Because protein motions are truly complex, the evaluation of the data even from such well-known techniques as neutron scattering (Magazu and Migliardo, 2011 [1]) and the Mossbauer effect (Chen and Yang, 2007 [2]) can lead to erroneous concepts and conclusions. We believe that notions such as the Lamb-Mossbauer relation, the protein dynamic transition, the protein glass transition, and the dynamic crossover are misleading or misapplied. To justify this statement we first briefly describe our view of dynamic proteins and then explain why we believe that these notions should be revised or abandoned. (C) 2013 Elsevier B.V. All rights reserved. C1 [Fenimore, Paul W.; Frauenfelder, Hans; McMahon, Benjamin H.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Magazu, Salvatore; Migliardo, Federica] Univ Messina, Dept Phys & Earth Sci, I-98166 Messina, Italy. [Mezei, Ferenc] European Spallat Source ESS AB, Lund, Sweden. [Young, Robert D.] Arizona State Univ, Tempe, AZ 85287 USA. [Stroe, Izabela] Worcester Polytech Inst, Worcester, MA 01609 USA. RP Fenimore, PW (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM paulf@lanl.gov NR 49 TC 13 Z9 13 U1 2 U2 43 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0301-0104 EI 1873-4421 J9 CHEM PHYS JI Chem. Phys. PD OCT 16 PY 2013 VL 424 BP 2 EP 6 DI 10.1016/j.chemphys.2013.06.023 PG 5 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 252DA UT WOS:000326983700002 ER PT J AU Nickels, JD AF Nickels, Jonathan D. TI Instrumental resolution effects in neutron scattering studies of protein dynamics SO CHEMICAL PHYSICS LA English DT Article DE Neutron scattering; GFP; Protein dynamics; Instrumental resolution; Data treatment ID GREEN FLUORESCENT PROTEIN; HYDRATION WATER; MOLECULAR MOTIONS; TRANSITION; SPECTROSCOPY; SOLVENT; GLASSES; SOFT; GFP AB In this study, the dynamics of Green Fluorescent protein (GFP) are analyzed using three neutron scattering spectrometers. We focus on the effect of instrumental energy resolution in the analysis of the elastic incoherent structure factor (EISF) and mean square displacement (MSD). This topic still remains a source of controversy. Our data clearly demonstrate the presence of the resolution effect in the dynamic transition for hydrated protein and the onset of translational motions in hydration water consistent with previous results from quasielastic neutron scattering. The 190 K onset of motions in hydration water observed at similar to 1 ns is also consistent with a T-g of hydration water below 190 K. (C) 2012 Elsevier B. V. All rights reserved. C1 [Nickels, Jonathan D.] Oak Ridge Natl Lab, Joint Inst Neutron Sci, Oak Ridge, TN 37831 USA. [Nickels, Jonathan D.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. RP Nickels, JD (reprint author), Oak Ridge Natl Lab, Joint Inst Neutron Sci, POB 2008,MS 6453,Bldg 8630,Suite B201, Oak Ridge, TN 37831 USA. EM jnickels@ornl.gov RI Nickels, Jonathan/I-1913-2012 OI Nickels, Jonathan/0000-0001-8351-7846 FU Department of Energy through the Experimental Program to Stimulate Competitive Research program [DE-FG02-08ER46528]; Spallation Neutron Source through UT-Battelle FX Thanks to Alexei Sokolov for many helpful discussions and to Hugh M. O'Neill, Qiu Zhang, Kevin L. Weiss, Eugene Mamontov, Georg Ehlers, and Madhusudan Tyagi for their help with samples and measurements. The author acknowledges Department of Energy support through the Experimental Program to Stimulate Competitive Research program (Grant No. DE-FG02-08ER46528) and support from Spallation Neutron Source through UT-Battelle. NR 40 TC 4 Z9 4 U1 2 U2 16 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0301-0104 EI 1873-4421 J9 CHEM PHYS JI Chem. Phys. PD OCT 16 PY 2013 VL 424 BP 7 EP 11 DI 10.1016/j.chemphys.2012.11.021 PG 5 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 252DA UT WOS:000326983700003 ER PT J AU Mamontov, E O'Neill, H Zhang, Q Chathoth, SM AF Mamontov, E. O'Neill, H. Zhang, Q. Chathoth, S. M. TI Temperature dependence of the internal dynamics of a protein in an aqueous solvent: Decoupling from the solvent viscosity SO CHEMICAL PHYSICS LA English DT Article DE Protein; Water; Solution; Dynamics; Neutron scattering ID NEUTRON-SCATTERING; SECONDARY STRUCTURE; GLASS-TRANSITION; HYDRATION WATER; ENZYME-ACTIVITY; HYDROGEN-BONDS; LIQUID WATER; FLUCTUATIONS; MYOGLOBIN; LICL AB We have recently observed decoupling of the dynamics of a protein from its aqueous solvent [Chu et al., JPCL 3 (2012) 380]; here we report the more detailed studies. We analyzed quasielastic neutron scattering data from a 40 mg/ml solution of lysozyme in (D2O)(8)(LiCl) and (H2O)(8)(LiCl). The internal dynamics of lysozyme exhibited super-Arrhenius temperature dependence with no crossover to a different regime down to at least 200 K. The decoupling of the internal protein dynamics from the viscosity of its aqueous solvent is evident. The temperature dependence of the protein dynamics indicates an apparent dynamic arrest at a temperature above 190 K, whereas the glass transition temperature for the solvent is around 135-140 K. The internal dynamics of the solvated protein is coupled to the dynamics of its hydration shell, not of the bulk solvent, which is qualitatively altered by the salt to defer the dynamic arrest to 135-140 K. (C) 2013 Elsevier B. V. All rights reserved. C1 [Mamontov, E.; Chathoth, S. M.] Oak Ridge Natl Lab, Neutron Sci Directorate, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. [O'Neill, H.; Zhang, Q.] Oak Ridge Natl Lab, Neutron Sci Directorate, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA. RP Mamontov, E (reprint author), Oak Ridge Natl Lab, Neutron Sci Directorate, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. EM mamontove@ornl.gov RI Mavila Chathoth, Suresh/E-7560-2010; Mamontov, Eugene/Q-1003-2015; OI Mavila Chathoth, Suresh/0000-0002-4120-6959; Mamontov, Eugene/0000-0002-5684-2675; O'Neill, Hugh/0000-0003-2966-5527 FU Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy (DOE); Office of Biological and Environmental Research, US DOE [ERKP291]; US DOE [DE-AC05-00OR22725] FX The neutron scattering experiments at Oak Ridge National Laboratory's (ORNL) Spallation Neutron Source were supported by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy (DOE). The authors acknowledge ORNL's Center for Structural Molecular Biology (Project ERKP291) supported by the Office of Biological and Environmental Research, US DOE. ORNL is managed by UTBattelle, LLC, for the US DOE under Contract No. DE-AC05-00OR22725. NR 45 TC 3 Z9 3 U1 2 U2 19 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0301-0104 EI 1873-4421 J9 CHEM PHYS JI Chem. Phys. PD OCT 16 PY 2013 VL 424 BP 12 EP 19 DI 10.1016/j.chemphys.2013.02.026 PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 252DA UT WOS:000326983700004 ER PT J AU Weber, JKR Benmore, CJ Tailor, AN Tumber, SK Neuefeind, J Cherry, B Yarger, JL Mou, Q Weber, W Byrn, SR AF Weber, J. K. R. Benmore, C. J. Tailor, A. N. Tumber, S. K. Neuefeind, J. Cherry, B. Yarger, J. L. Mou, Q. Weber, W. Byrn, S. R. TI A neutron-X-ray, NMR and calorimetric study of glassy Probucol synthesized using containerless techniques SO CHEMICAL PHYSICS LA English DT Article DE Acoustic levitation; Amorphous pharmaceuticals; Liquids; Glass; X-ray; Neutron ID AMORPHOUS PHARMACEUTICAL SOLIDS; CHOLESTEROL-LOWERING DRUG; SCATTERING; STABILIZATION; LEVITATION; LIQUIDS AB Acoustic levitation was used to trap 1-3 mm diameter drops of Probucol and other pharmaceutical materials in containerless conditions. Samples were studied in situ using X-ray diffraction and ex situ using neutron diffraction, NMR and DSC techniques. The materials were brought into non-equilibrium states by supersaturating solutions or by supercooling melts. The glass transition and crystallization temperatures of glassy Probucol were 29 +/- 1 and 71 +/- 1 degrees C respectively. The glassy form was stable with a shelf life of at least 8 months. A neutron/X-ray difference function of the glass showed that while molecular sub-groups remain rigid, many of the hydrogen correlations observed in the crystal become smeared out in the disordered material. The glass is principally comprised of slightly distorted Form I Probucol molecules with disordered packing rather than large changes in the individual molecular structure. Avoiding surface contact-induced nucleation provided access to highly non-equilibrium phases and enabled synthesis of phase-pure glasses. (C) 2013 Elsevier B. V. All rights reserved. C1 [Weber, J. K. R.; Tailor, A. N.; Tumber, S. K.] Mat Dev Inc, Arlington Hts, IL 60004 USA. [Weber, J. K. R.; Benmore, C. J.] Argonne Natl Lab, Argonne, IL 60439 USA. [Benmore, C. J.; Yarger, J. L.; Weber, W.] Arizona State Univ, Dept Phys, Tempe, AZ 85287 USA. [Neuefeind, J.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Cherry, B.; Yarger, J. L.; Mou, Q.] Arizona State Univ, Magnet Resonance Res Ctr, Tempe, AZ 85287 USA. [Cherry, B.; Yarger, J. L.; Mou, Q.; Weber, W.] Arizona State Univ, Dept Chem & Biochem, Tempe, AZ 85287 USA. [Byrn, S. R.] Purdue Univ, Dept Ind & Phys Pharm, W Lafayette, IN 47907 USA. RP Weber, JKR (reprint author), Mat Dev Inc, Arlington Hts, IL 60004 USA. EM rweber@anl.gov RI Neuefeind, Joerg/D-9990-2015; Yarger, Jeff/L-8748-2014; OI Neuefeind, Joerg/0000-0002-0563-1544; Yarger, Jeff/0000-0002-7385-5400; Benmore, Chris/0000-0001-7007-7749 FU US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; National Nuclear Security Administration Carnegie/DOE Alliance Center (NNSA CDAC) [DE-FC52-08NA28554]; US National Science Foundation (NSF), Chemistry Division (CHE) [CHE-1011937] FX This research was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under contract DE-AC02-06CH11357. We would like to thank Rick Spence at the Advanced Photon Source for his help in setting up the levitator equipment. JLY would like to acknowledge support from the National Nuclear Security Administration Carnegie/DOE Alliance Center (NNSA CDAC) Grant number DE-FC52-08NA28554 and the US National Science Foundation (NSF), Chemistry Division (CHE) under Grant CHE-1011937. NR 22 TC 6 Z9 6 U1 2 U2 20 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0301-0104 EI 1873-4421 J9 CHEM PHYS JI Chem. Phys. PD OCT 16 PY 2013 VL 424 BP 89 EP 92 DI 10.1016/j.chemphys.2013.05.019 PG 4 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 252DA UT WOS:000326983700017 ER PT J AU Alarcon, R Balascuta, S Benson, SV Bertozzi, W Boyce, JR Cowan, R Douglas, D Evtushenko, P Fisher, P Ihloff, E Kalantarians, N Kelleher, A Legg, R Milner, RG Neil, GR Ou, L Schmookler, B Tennant, C Tschalar, C Williams, GP Zhang, S AF Alarcon, R. Balascuta, S. Benson, S. V. Bertozzi, W. Boyce, J. R. Cowan, R. Douglas, D. Evtushenko, P. Fisher, P. Ihloff, E. Kalantarians, N. Kelleher, A. Legg, R. Milner, R. G. Neil, G. R. Ou, L. Schmookler, B. Tennant, C. Tschalaer, C. Williams, G. P. Zhang, S. TI Transmission of Megawatt Relativistic Electron Beams through Millimeter Apertures SO PHYSICAL REVIEW LETTERS LA English DT Article ID INTERNAL GAS-TARGET; FLUKA CODE; RADIATION AB High-power, relativistic electron beams from energy-recovering linacs have great potential to realize new experimental paradigms for pioneering innovation in fundamental and applied research. A major design consideration for this new generation of experimental capabilities is the understanding of the halo associated with these bright, intense beams. In this Letter, we report on measurements performed using the 100 MeV, 430 kW cw electron beam from the energy-recovering linac at the Jefferson Laboratory's Free Electron Laser facility as it traversed a set of small apertures in a 127 mm long aluminum block. Thermal measurements of the block together with neutron measurements near the beam-target interaction point yielded a consistent understanding of the beam losses. These were determined to be 3 ppm through a 2 mm diameter aperture and were maintained during a 7 h continuous run. C1 [Bertozzi, W.; Cowan, R.; Fisher, P.; Ihloff, E.; Kelleher, A.; Milner, R. G.; Ou, L.; Schmookler, B.; Tschalaer, C.] MIT, Nucl Sci Lab, Cambridge, MA 02139 USA. [Benson, S. V.; Boyce, J. R.; Douglas, D.; Evtushenko, P.; Legg, R.; Neil, G. R.; Tennant, C.; Williams, G. P.; Zhang, S.] Thomas Jefferson Natl Accelerator Facil, Free Electron Laser Grp, Newport News, VA 23606 USA. [Kalantarians, N.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Alarcon, R.; Balascuta, S.] Arizona State Univ, Dept Phys, Tempe, AZ 85287 USA. RP Alarcon, R (reprint author), Arizona State Univ, Dept Phys, Tempe, AZ 85287 USA. RI Balascuta, Septimiu/J-7679-2015 OI Balascuta, Septimiu/0000-0003-2331-294X FU United States Department of Energy Office of Science (High Energy and Nuclear Physics) FX We gratefully acknowledge the outstanding efforts of both the staff of the Jefferson Laboratory to deliver the high quality FEL beam and the staff of the MIT-Bates Research and Engineering Center who designed, constructed, and delivered the test target assembly. We thank the referees of this Letter for their thoughtful and constructive criticism. This research is supported by the United States Department of Energy Office of Science (High Energy and Nuclear Physics). NR 22 TC 0 Z9 0 U1 0 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 16 PY 2013 VL 111 IS 16 AR 164801 DI 10.1103/PhysRevLett.111.164801 PG 5 WC Physics, Multidisciplinary SC Physics GA 241DW UT WOS:000326147600009 PM 24182271 ER PT J AU Trugman, DT Daub, EG Guyer, RA Johnson, PA AF Trugman, Daniel T. Daub, Eric G. Guyer, Robert A. Johnson, Paul A. TI Modeling dynamic triggering of tectonic tremor using a brittle-ductile friction model SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE tectonic tremor; dynamic triggering; tremor; triggering ID NON-VOLCANIC TREMOR; SAN-ANDREAS FAULT; NONVOLCANIC TREMOR; EPISODIC TREMOR; STRESS TRANSFER; EARTHQUAKE; SLIP; SUBDUCTION; TRANSIENT; JAPAN AB We study the physics of dynamically triggered tectonic tremor by applying a brittle-ductile friction model in which we conceptualize the tremor source as a rigid block subject to driving and frictional forces. To simulate dynamic triggering of tremor, we apply a stress perturbation that mimics the surface waves of remote earthquakes. The tectonic and wave perturbation stresses define a phase space that demonstrates that both the timing and amplitude of the dynamic perturbations control the fundamental characteristics of triggered tremor. Tremor can be triggered instantaneously or with a delayed onset if the dynamic perturbation significantly alters the frictional state of the tremor source. C1 [Trugman, Daniel T.; Guyer, Robert A.; Johnson, Paul A.] Los Alamos Natl Lab, Solid Earth Geophys Grp, Los Alamos, NM 87545 USA. [Daub, Eric G.] Univ Grenoble 1, Inst Sci Terre, Grenoble, France. [Guyer, Robert A.] Univ Nevada, Dept Phys, Reno, NV 89557 USA. RP Trugman, DT (reprint author), Los Alamos Natl Lab, Solid Earth Geophys Grp, POB 1663, Los Alamos, NM 87545 USA. EM dtrugman@lanl.gov OI Johnson, Paul/0000-0002-0927-4003; Trugman, Daniel/0000-0002-9296-4223 NR 33 TC 3 Z9 3 U1 0 U2 11 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD OCT 16 PY 2013 VL 40 IS 19 BP 5075 EP 5079 DI 10.1002/grl.50981 PG 5 WC Geosciences, Multidisciplinary SC Geology GA 243JB UT WOS:000326311600019 ER PT J AU Lipschutz, MI Yang, XZ Chatterjee, R Tilley, TD AF Lipschutz, Michael I. Yang, Xinzheng Chatterjee, Ruchira Tilley, T. Don TI A Structurally Rigid Bis(amido) Ligand Framework in Low-Coordinate Ni(I), Ni(II), and Ni(III) Analogues Provides Access to a Ni(III) Methyl Complex via Oxidative Addition SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID AMIDO COMPLEXES; 2-COORDINATE; NICKEL; ALKYL; REACTIVITY; CATALYST AB A structurally persistent bis-amido ligand framework capable of supporting nickel compounds in three different oxidation states has been identified. A highly unusual, isolable Ni(III) alkyl species has been prepared and characterized via a rare example of a two-electron oxidative addition of MeI to Ni(I). C1 [Lipschutz, Michael I.; Tilley, T. Don] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Yang, Xinzheng] Univ Calif Berkeley, Mol Graph & Computat Facil, Berkeley, CA 94720 USA. [Yang, Xinzheng] Chinese Acad Sci, Inst Chem, Beijing 100190, Peoples R China. [Chatterjee, Ruchira] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Tilley, TD (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM tdtdley@berkeley.edu RI Yang, Xinzheng/F-6893-2010 OI Yang, Xinzheng/0000-0002-2036-1220 FU National Science Foundation [CHE-1265674, CHE-0840505] FX This work was funded by the National Science Foundation under grant no. CHE-1265674. The Molecular Graphics and Computational facility (College of Chemistry, University of California, Berkeley) is supported by the National Science Foundation under grant no. CHE-0840505. NR 29 TC 37 Z9 37 U1 2 U2 46 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD OCT 16 PY 2013 VL 135 IS 41 BP 15298 EP 15301 DI 10.1021/ja408151h PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA 240VG UT WOS:000326125200008 PM 24079707 ER PT J AU Zhai, DY Wang, HH Yang, JB Lau, KC Li, KX Amine, K Curtiss, LA AF Zhai, Dengyun Wang, Hsien-Hau Yang, Junbing Lau, Kah Chun Li, Kaixi Amine, Khalil Curtiss, Larry A. TI Disproportionation in Li-O-2 Batteries Based on a Large Surface Area Carbon Cathode SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID LITHIUM-OXYGEN BATTERIES; AIR BATTERIES; ELECTROLYTES; REDUCTION; ELECTROCHEMISTRY; PERFORMANCE; ELECTRODES; MECHANISM; CATALYSTS; KINETICS AB In this paper we report on a kinetics study of the discharge process and its relationship to the charge overpotential in a Li-O-2 cell for large surface area cathode material. The kinetics study reveals evidence for a first-order disproportionation reaction during discharge from an oxygen-rich Li2O2 component with superoxide-like character to a Li2O2 component. The oxygen-rich superoxide-like component has a much smaller potential during charge (3.2-3.5 V) than the Li2O2 component (similar to 4.2 V). The formation of the superoxide-like component is likely due to the porosity of the activated carbon used in the Li-O-2 cell cathode that provides a good environment for growth during discharge. The discharge product containing these two components is characterized by toroids, which are assemblies of nanoparticles. The morphologic growth and decomposition process of the toroids during the reversible discharge/charge process was observed by scanning electron microscopy and is consistent with the presence of the two components in the discharge product. The results of this study provide new insight into how growth conditions control the nature of discharge product, which can be used to achieve improved performance in Li-O-2 cell. C1 [Zhai, Dengyun; Yang, Junbing; Amine, Khalil] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Wang, Hsien-Hau; Lau, Kah Chun; Curtiss, Larry A.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Li, Kaixi] Chinese Acad Sci, Inst Coal Chem, Key Lab Carbon Mat, Taiyuan 030001, Shanxi, Peoples R China. [Amine, Khalil] King Abdulazi Univ, Jeddah 21589, Saudi Arabia. RP Amine, K (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM amine@anl.gov; curtiss@anl.gov RI Lau, Kah Chun/A-9348-2013 OI Lau, Kah Chun/0000-0002-4925-3397 FU U.S. Department of Energy, Joint Center for Energy Storage Research and Vehicle Technologies Office by UChicago Argonne, LLC [DE-AC02-06CH11357] FX Research at Argonne National Laboratory was funded by the U.S. Department of Energy, Joint Center for Energy Storage Research and Vehicle Technologies Office under Contract No. DE-AC02-06CH11357 by UChicago Argonne, LLC. The electron microscopy measurement was accomplished at the Electron Microscopy Center for Materials Research, and the Raman measurements were performed at the Center for Nanoscale Materials at Argonne National Laboratory. We also acknowledge helpful discussions with Professor Linda Nazar. NR 40 TC 124 Z9 126 U1 17 U2 188 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 EI 1520-5126 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD OCT 16 PY 2013 VL 135 IS 41 BP 15364 EP 15372 DI 10.1021/ja403199d PG 9 WC Chemistry, Multidisciplinary SC Chemistry GA 240VG UT WOS:000326125200023 PM 24053681 ER PT J AU Xu, CF Liu, R Mehta, AK Guerrero-Ferreira, RC Wright, ER Dunin-Horkawicz, S Morris, K Serpell, LC Zuo, XB Wall, JS Conticello, VP AF Xu, Chunfu Liu, Rui Mehta, Anil K. Guerrero-Ferreira, Ricardo C. Wright, Elizabeth R. Dunin-Horkawicz, Stanislaw Morris, Kyle Serpell, Louise C. Zuo, Xiaobing Wall, Joseph S. Conticello, Vincent P. TI Rational Design of Helical Nanotubes from Self-Assembly of Coiled-Coil Lock Washers SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID TRANSMISSION ELECTRON-MICROSCOPY; DE-NOVO DESIGN; CYCLODEXTRIN INCLUSION COMPLEXES; DOUBLE-RESONANCE NMR; BETA-SHEET PEPTIDE; BIOLOGICAL MACROMOLECULES; PULSE IMPERFECTIONS; SOLUTION SCATTERING; ORGANIC NANOTUBES; FLUORESCENT-PROBE AB Design of a structurally defined helical assembly is described that involves recoding of the amino acid sequence of peptide GCN4-pAA. In solution and the crystalline state, GCN4-pAA adopts a 7-helix bundle structure that resembles a supramolecular lock washer. Structurally informed mutagenesis of the sequence of GCN4-pAA afforded peptide 7HSAP1, which undergoes self-association into a nanotube via noncovalent interactions between complementary interfaces of the coiled-coil lock-washer structures. Biophysical measurements conducted in solution and the solid state over multiple length scales of structural hierarchy are consistent with self-assembly of nanotube structures derived from 7-helix bundle subunits. The dimensions of the supramolecular assemblies are similar to those observed in the crystal structure of GCN4-pAA. Fluorescence studies of the interaction of 7HSAP1 with the solvatochromic fluorophore PRODAN indicated that the nanotubes could encapsulate shape-appropriate small molecules with high binding affinity. C1 [Xu, Chunfu; Liu, Rui; Mehta, Anil K.; Conticello, Vincent P.] Emory Univ, Dept Chem, Atlanta, GA 30322 USA. [Guerrero-Ferreira, Ricardo C.; Wright, Elizabeth R.] Emory Univ, Sch Med, Dept Pediat, Div Pediat Infect Dis,Childrens Healthcare Atlant, Atlanta, GA 30322 USA. [Dunin-Horkawicz, Stanislaw] Int Inst Mol & Cell Biol, Lab Bioinformat & Prot Engn, PL-02109 Warsaw, Poland. [Morris, Kyle; Serpell, Louise C.] Univ Sussex, Sch Life Sci, Falmer BN1 9QG, E Sussex, England. [Zuo, Xiaobing] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. [Wall, Joseph S.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Conticello, VP (reprint author), Emory Univ, Dept Chem, 1515 Dickey Dr, Atlanta, GA 30322 USA. EM vcontic@emory.edu OI Guerrero-Ferreira, Ricardo/0000-0002-3664-8277; Conticello, Vincent/0000-0001-6940-6947; Mehta, Anil/0000-0002-9867-151X; Serpell, Louise/0000-0001-9335-7751; Zuo, Xiaobing/0000-0002-0134-4804 FU NSF [CHE-1012620, 0923395, CHE-0131013]; Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-ER15377]; Emory University, Children's Healthcare of Atlanta; Center for AIDS Research at Emory University [P30 AI050409]; Georgia Research Alliance; US DOE Office of Basic Energy Sciences, Division of Material Sciences [W-31-109-Eng-38] FX V.P.C. would like to dedicate this article to Professor David Tirrell on the occasion of his 60th birthday. We thank Stefan Lutz for use of the spectrofluorimeter. Gevorg Grigoryan is acknowledged for advice on the use of the program CCCP. V.P.C. acknowledges financial support from NSF (CHE-1012620) for peptide synthesis and preliminary structural characterization and the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the U.S. Department of Energy through Grant (DE-ER15377) for solid-state NMR and electron microscopy. This work was supported in part by Emory University, Children's Healthcare of Atlanta, the Center for AIDS Research at Emory University (P30 AI050409), and the Georgia Research Alliance to E.R.W. and NSF grant 0923395 to E.R.W. This work benefited from the use of the APS funded by the US DOE Office of Basic Energy Sciences, Division of Material Sciences, under contract W-31-109-Eng-38. Electron microscopy was performed with equipment housed in and the support of the Emory University Robert P. Apkarian Integrated Electron Microscopy Core. The circular dichroism spectropolarimeter was obtained from funds derived from NSF grant CHE-0131013. NR 114 TC 26 Z9 26 U1 10 U2 113 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD OCT 16 PY 2013 VL 135 IS 41 BP 15565 EP 15578 DI 10.1021/ja4074529 PG 14 WC Chemistry, Multidisciplinary SC Chemistry GA 240VG UT WOS:000326125200043 PM 24028069 ER PT J AU Breiten, B Lockett, MR Sherman, W Fujita, S Al-Sayah, M Lange, H Bowers, CM Heroux, A Krilov, G Whitesides, GM AF Breiten, Benjamin Lockett, Matthew R. Sherman, Woody Fujita, Shuji Al-Sayah, Mohammad Lange, Heiko Bowers, Carleen M. Heroux, Annie Krilov, Goran Whitesides, George M. TI Water Networks Contribute to Enthalpy/Entropy Compensation in Protein-Ligand Binding SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID INHOMOGENEOUS FLUID APPROACH; ENTROPY COMPENSATION; CARBONIC-ANHYDRASE; SOLVATION THERMODYNAMICS; SOLVENT REORGANIZATION; RECOGNITION; ENERGETICS; AFFINITY AB The mechanism (or mechanisms) of enthalpy-entropy (HIS) compensation in protein ligand binding remains controversial, and there are still no predictive models (theoretical or experimental) in which hypotheses of ligand binding can be readily tested. Here we describe a particularly well-defined system of protein and ligands-human carbonic anhydrase (HCA) and a series of benzothiazole sulfonamide ligands with different patterns of fluorination-that we use to define enthalpy/entropy (HIS) compensation in this system thermodynamically and structurally. The binding affinities of these ligands (with the exception of one ligand, in which the deviation is understood) to HCA are, despite differences in fluorination pattern, indistinguishable; they nonetheless reflect significant and compensating changes in enthalpy and entropy of binding. Analysis reveals that differences in the structure and thermodynamic properties of the waters surrounding the bound ligands are an important contributor to the observed H/S compensation. These results support the hypothesis that the molecules of water filling the active site of a protein, and surrounding the ligand, are as important as the contact interactions between the protein and the ligand for biomolecular recognition, and in determining the thermodynamics of binding. C1 [Breiten, Benjamin; Lockett, Matthew R.; Fujita, Shuji; Al-Sayah, Mohammad; Lange, Heiko; Bowers, Carleen M.; Whitesides, George M.] Harvard Univ, Dept Chem & Chem Biol, Cambridge, MA 02138 USA. [Sherman, Woody; Krilov, Goran] Schrodinger Inc, New York, NY 10036 USA. [Heroux, Annie] Brookhaven Natl Lab, Natl Synchrotron Light Source, Upton, NY 11973 USA. [Whitesides, George M.] Harvard Univ, Wyss Inst Biol Inspired Engn, Cambridge, MA 02138 USA. RP Whitesides, GM (reprint author), Harvard Univ, Dept Chem & Chem Biol, 12 Oxford St, Cambridge, MA 02138 USA. EM gwhitesides@gmwgroup.harvard.edu RI Lockett, Matthew/A-6020-2015; OI Lockett, Matthew/0000-0003-4851-7757; Al-Sayah, Mohammad/0000-0001-6321-0556; Lange, Heiko/0000-0003-3845-7017 FU National Science Foundation [NSF CHE-1152196]; Wyss Institute for Biologically Inspired Engineering; Arab Fund Fellowship Program (AFFP); American University of Sharjah (UAE); German Research Foundation (DFG) FX The authors acknowledge Drs. Demetri T. Moustakas, Philip W. Snyder, Dmitrji Rappoport, and Mr. Jang Moon Yoon for their technical contributions and useful conversations. This work was supported by the National Science Foundation (NSF CHE-1152196) and the Wyss Institute for Biologically Inspired Engineering. MA. thanks the Arab Fund Fellowship Program (AFFP) and the American University of Sharjah (UAE) for a visiting scholar stipend award. H.L. thanks the German Research Foundation (DFG) for a postdoctoral research stipend. NR 32 TC 83 Z9 84 U1 2 U2 100 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 EI 1520-5126 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD OCT 16 PY 2013 VL 135 IS 41 BP 15579 EP 15584 DI 10.1021/ja4075776 PG 6 WC Chemistry, Multidisciplinary SC Chemistry GA 240VG UT WOS:000326125200044 PM 24044696 ER PT J AU Akhanjee, S Tsuchiizu, M Furusaki, A AF Akhanjee, Shimul Tsuchiizu, Masahisa Furusaki, Akira TI Composite pairing and superfluidity in a one-dimensional resonant Bose-Fermi mixture SO PHYSICAL REVIEW A LA English DT Article ID ULTRACOLD GASES; 2-BAND MODEL; QUANTUM; SYSTEMS; BOSONS AB We study the ground-state properties of one-dimensional mixtures of bosonic and fermionic atoms resonantly coupled to fermionic Feshbach molecules. When the particle densities of fermionic atoms and Feshbach molecules differ, the system undergoes various depletion transitions between binary and ternary mixtures as a function of the detuning parameter. However, when the particle densities of fermionic atoms and Feshbach molecules are identical, the molecular conversion and disassociation processes induce a gap in a sector of low-energy excitations, and the remaining system can be described by a two-component Tomonaga-Luttinger liquid. Using a bosonization scheme, we derive the effective low-energy Hamiltonian for the system, which has a similar form as that of the two-chain problem of coupled Tomonaga-Luttinger liquids. With the help of improved perturbative renormalization group analysis of the latter problem, we determine the ground-state phase diagram and find that it contains a phase dominated by composite superfluid or pairing correlations between the open and closed resonant channels. C1 [Akhanjee, Shimul; Furusaki, Akira] RIKEN, Condensed Matter Theory Lab, Wako, Saitama 3510198, Japan. [Akhanjee, Shimul] Brookhaven Natl Lab, Dept Condensed Matter Phys & Mat Sci, Upton, NY 11973 USA. [Tsuchiizu, Masahisa] Nagoya Univ, Dept Phys, Nagoya, Aichi 4648602, Japan. [Furusaki, Akira] RIKEN, CEMS, Wako, Saitama 3510198, Japan. RP Akhanjee, S (reprint author), RIKEN, Condensed Matter Theory Lab, 2-1 Hirosawa, Wako, Saitama 3510198, Japan. RI Furusaki, Akira/B-3204-2008 OI Furusaki, Akira/0000-0001-8394-0003 FU RIKEN FPR program FX We thank T. Giamarchi, E. Orignac, and Masahiro Sato for important discussions. S.A. acknowledges helpful conversations with A. M. Tsvelik and support from the RIKEN FPR program. NR 52 TC 0 Z9 0 U1 0 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1050-2947 EI 1094-1622 J9 PHYS REV A JI Phys. Rev. A PD OCT 16 PY 2013 VL 88 IS 4 AR 043620 DI 10.1103/PhysRevA.88.043620 PG 14 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA 240ED UT WOS:000326076600012 ER PT J AU Kehayias, P Doherty, MW English, D Fischer, R Jarmola, A Jensen, K Leefer, N Hemmer, P Manson, NB Budker, D AF Kehayias, P. Doherty, M. W. English, D. Fischer, R. Jarmola, A. Jensen, K. Leefer, N. Hemmer, P. Manson, N. B. Budker, D. TI Infrared absorption band and vibronic structure of the nitrogen-vacancy center in diamond SO PHYSICAL REVIEW B LA English DT Article ID NANOSCALE RESOLUTION; SPINS AB Negatively charged nitrogen-vacancy (NV-) color centers in diamond have generated much interest for use in quantum technology. Despite the progress made in developing their applications, many questions about the basic properties of NV- centers remain unresolved. Understanding these properties can validate theoretical models of NV-, improve their use in applications, and support their development into competitive quantum devices. In particular, knowledge of the phonon modes of the (1)A(1) electronic state is key for understanding the optical pumping process. Using pump-probe spectroscopy, we measured the phonon sideband of the E-1 -> (1)A(1) electronic transition in the NV- center. From this we calculated the E-1 -> (1)A(1) one-phonon absorption spectrum and found it to differ from that of the E-3 -> (3)A(2) transition, a result which is not anticipated by previous group-theoretical models of the NV- electronic states. We identified a high-energy 169-meV localized phonon mode of the (1)A(1) level. C1 [Kehayias, P.; English, D.; Jarmola, A.; Jensen, K.; Leefer, N.; Budker, D.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Doherty, M. W.; Manson, N. B.] Australian Natl Univ, RSPE, Laser Phys Ctr, Canberra, ACT 0200, Australia. [Fischer, R.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Hemmer, P.] Texas A&M Univ, Dept Elect & Comp Engn, College Stn, TX 77843 USA. [Budker, D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. RP Kehayias, P (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM pkehayias@berkeley.edu; budker@berkeley.edu RI Doherty, Marcus/O-1222-2013; Budker, Dmitry/F-7580-2016; Jensen, Kasper/P-8359-2014; OI Doherty, Marcus/0000-0002-5473-6481; Budker, Dmitry/0000-0002-7356-4814; Jensen, Kasper/0000-0002-8417-4328; Leefer, Nathan/0000-0002-4940-8432; Kehayias, Pauli/0000-0002-7597-4358 FU NSF; DOE SCGF; AFOSR/DARPA QuASAR program; NATO SFP; IMOD; ARC [DP120102232]; Danish Council for Independent Research in Natural Sciences FX We are grateful to the group of Professor F. Wang (UC Berkeley) for help with the supercontinuum laser. We thank V. Acosta and C. Santori (Hewlett-Packard Laboratories), and V. Huxter and S. Choi (UC Berkeley) for useful discussions. This work was supported by the NSF, DOE SCGF, the AFOSR/DARPA QuASAR program, NATO SFP, IMOD, ARC (DP120102232), and the Danish Council for Independent Research in Natural Sciences. NR 41 TC 13 Z9 13 U1 2 U2 39 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 16 PY 2013 VL 88 IS 16 AR 165202 DI 10.1103/PhysRevB.88.165202 PG 5 WC Physics, Condensed Matter SC Physics GA 240FU UT WOS:000326081200002 ER PT J AU Mardegan, JRL Fabbris, G Veiga, LSI Adriano, C Avila, MA Haskel, D Giles, C AF Mardegan, J. R. L. Fabbris, G. Veiga, L. S. I. Adriano, C. Avila, M. A. Haskel, D. Giles, C. TI Pressure-induced amorphization and collapse of magnetic order in the type-I clathrate Eu8Ga16Ge30 SO PHYSICAL REVIEW B LA English DT Article ID CRYSTAL-STRUCTURE; THERMOELECTRIC-MATERIALS; CIRCULAR-DICHROISM; SR8GA16GE30; BA8GA16GE30; UFE4P12; HEAT; GE AB We investigate the low temperature structural and electronic properties of the type-I clathrate Eu8Ga16Ge30 under pressure using x-ray powder diffraction (XRD), x-ray absorption near-edge structure (XANES), and x-ray magnetic circular dichroism (XMCD) techniques. The XRD measurements reveal a transition to an amorphous phase above 18 GPa. Unlike previous reports on other clathrate compounds, no volume collapse is observed prior to the crystalline-amorphous phase transition which takes place when the unit cell volume is reduced to 81% of its ambient pressure value. Fits of the pressure-dependent relative volume to a Murnaghan equation of state yield a bulk modulus B-0 = 65 +/- 3 GPa and a pressure derivative B '(0) = 3.3 +/- 0.5. The Eu L2-edge XMCD data shows quenching of the magnetic order at a pressure coincident with the crystalline-amorphous phase transition. This information along with the persistence of an Eu2+ valence state observed in the XANES spectra up to the highest pressure point (22 GPa) indicates that the suppression of XMCD intensity is due to the loss of long range magnetic order. When compared with other clathrates, the results point to the importance of guest ion-cage interactions in determining the mechanical stability of the framework structure and the critical pressure for amorphization. Finally, the crystalline structure is not found to recover after pressure release, resulting in an amorphous material that is at least metastable at ambient pressure and temperature. C1 [Mardegan, J. R. L.; Veiga, L. S. I.; Adriano, C.; Giles, C.] Univ Estadual Campinas, Inst Fis Gleb Wataghin, BR-13083859 Sao Paulo, Brazil. [Mardegan, J. R. L.; Fabbris, G.; Haskel, D.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Fabbris, G.] Washington Univ, Dept Phys, St Louis, MO 63130 USA. [Veiga, L. S. I.] Lab Nacl Luz Sincrotron, BR-13083970 Campinas, SP, Brazil. [Avila, M. A.] UFABC, CCNH, BR-09210580 Sao Paulo, Brazil. RP Mardegan, JRL (reprint author), Univ Estadual Campinas, Inst Fis Gleb Wataghin, BR-13083859 Sao Paulo, Brazil. EM giles@ifi.unicamp.br RI Fabbris, Gilberto/F-3244-2011; Avila, Marcos/B-3578-2008; Inst. of Physics, Gleb Wataghin/A-9780-2017 OI Fabbris, Gilberto/0000-0001-8278-4985; Avila, Marcos/0000-0002-3796-3244; FU FAPESP (SP-Brazil) [2009/10264-0, 2011/24166-0, 2012/10675-2, 2012/17562-9]; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC-02-06CH11357] FX This work was supported by FAPESP (SP-Brazil) under Contracts No. 2009/10264-0, No. 2011/24166-0, No. 2012/10675-2, and No. 2012/17562-9. Work at Argonne is supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC-02-06CH11357. We would like to thank Curtis Kenny-Benson and Dmitry Popov for their assistance at 16-BMD beamline, Sergey N. Tkachev for the gas loading, and P. F. S. Rosa and W. Iwamoto for assistance in sample preparation. We also thank the GSECARS group for use of the gas loading and laser drilling facilities. NR 62 TC 5 Z9 5 U1 0 U2 25 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 16 PY 2013 VL 88 IS 14 AR 144105 DI 10.1103/PhysRevB.88.144105 PG 8 WC Physics, Condensed Matter SC Physics GA 240FP UT WOS:000326080700001 ER PT J AU Recchia, F Chiara, CJ Janssens, RVF Weisshaar, D Gade, A Walters, WB Albers, M Alcorta, M Bader, VM Baugher, T Bazin, D Berryman, JS Bertone, PF Brown, BA Campbell, CM Carpenter, MP Chen, J Crawford, HL David, HM Doherty, DT Hoffman, CR Kondev, FG Korichi, A Langer, C Larson, N Lauritsen, T Liddick, SN Lunderberg, E Macchiavelli, AO Noji, S Prokop, C Rogers, AM Seweryniak, D Stroberg, SR Suchyta, S Williams, S Wimmer, K Zhu, S AF Recchia, F. Chiara, C. J. Janssens, R. V. F. Weisshaar, D. Gade, A. Walters, W. B. Albers, M. Alcorta, M. Bader, V. M. Baugher, T. Bazin, D. Berryman, J. S. Bertone, P. F. Brown, B. A. Campbell, C. M. Carpenter, M. P. Chen, J. Crawford, H. L. David, H. M. Doherty, D. T. Hoffman, C. R. Kondev, F. G. Korichi, A. Langer, C. Larson, N. Lauritsen, T. Liddick, S. N. Lunderberg, E. Macchiavelli, A. O. Noji, S. Prokop, C. Rogers, A. M. Seweryniak, D. Stroberg, S. R. Suchyta, S. Williams, S. Wimmer, K. Zhu, S. TI Configuration mixing and relative transition rates between low-spin states in Ni-68 SO PHYSICAL REVIEW C LA English DT Article ID CORE-EXCITED STATES; GRETINA; ARRAY AB The low-spin level scheme of Ni-68 was investigated following two-neutron-knockout and multinucleon-transferreactions. The energy of the first excited state was determined to be E-x(0(2)(+)) = 1603.5(3) keV. Relative B(E2) transition probabilities were deduced and compared with shell-model calculations using several modern effective interactions. Theory reproduces the data well, but indicates substantial mixing of multi-particle, multi-hole configurations for the lowest observed 0(+) and 2(+) states. C1 [Recchia, F.; Weisshaar, D.; Gade, A.; Bader, V. M.; Baugher, T.; Bazin, D.; Berryman, J. S.; Brown, B. A.; Langer, C.; Larson, N.; Liddick, S. N.; Lunderberg, E.; Noji, S.; Prokop, C.; Stroberg, S. R.; Suchyta, S.; Williams, S.; Wimmer, K.] Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA. [Chiara, C. J.; Walters, W. B.] Univ Maryland, Dept Chem & Biochem, College Pk, MD 20742 USA. [Chiara, C. J.; Janssens, R. V. F.; Albers, M.; Alcorta, M.; Bertone, P. F.; Carpenter, M. P.; David, H. M.; Doherty, D. T.; Hoffman, C. R.; Korichi, A.; Lauritsen, T.; Rogers, A. M.; Seweryniak, D.; Zhu, S.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Gade, A.; Bader, V. M.; Baugher, T.; Bertone, P. F.; Brown, B. A.; Lunderberg, E.; Stroberg, S. R.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Campbell, C. M.; Crawford, H. L.; Macchiavelli, A. O.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Chen, J.; Kondev, F. G.] Argonne Natl Lab, Nucl Engn Div, Argonne, IL 60439 USA. [David, H. M.; Doherty, D. T.] Univ Edinburgh, Sch Phys & Astron, Edinburgh EH9 3JZ, Midlothian, Scotland. [Korichi, A.] CNRS, CSNSM, IN2P3, F-91405 Orsay, France. [Larson, N.; Liddick, S. N.; Prokop, C.; Suchyta, S.] Michigan State Univ, Dept Chem Engn, E Lansing, MI 48824 USA. [Wimmer, K.] Cent Michigan Univ, Dept Phys, Mt Pleasant, MI 48859 USA. RP Recchia, F (reprint author), Univ Padua, Dipartimento Fis & Astron Galileo Galilei, I-35131 Padua, Italy. RI Gade, Alexandra/A-6850-2008; Alcorta, Martin/G-7107-2011; Langer, Christoph/D-5490-2014; Carpenter, Michael/E-4287-2015; Hoffman, Calem/H-4325-2016; Langer, Christoph/L-3422-2016; Larson, Nicole/S-5997-2016; OI Gade, Alexandra/0000-0001-8825-0976; Alcorta, Martin/0000-0002-6217-5004; Carpenter, Michael/0000-0002-3237-5734; Hoffman, Calem/0000-0001-7141-9827; Larson, Nicole/0000-0003-0292-957X; Chen, Jun/0000-0003-0447-7466; Stroberg, Ragnar/0000-0002-0635-776X; Recchia, Francesco/0000-0002-8428-0112 FU US Department of Energy (DOE), Office of Nuclear Physics [DE-FG02-94-ER40834, DE-AC02-06CH11357]; National Science Foundation (NSF) [PHY-1102511]; DOE, National Nuclear Security Administration [DE-NA0000979]; DOE, Office of Science; NSF under Cooperative [PHY-1102511]; DOE [DE-AC02-05CH11231]; NSF [PHY-1068217] FX The authors thank J. P. Greene (ANL) for target preparation, I. Y. Lee (LBNL) and the GRETINA team for their efforts in making the array a reality, and the NSCL operations department. This work was supported in part by the US Department of Energy (DOE), Office of Nuclear Physics, under Grant No. DE-FG02-94-ER40834 and Contract No. DE-AC02-06CH11357, the National Science Foundation (NSF) under Contract No. PHY-1102511, and by the DOE, National Nuclear Security Administration, under Award No. DE-NA0000979. GRETINA was funded by the DOE, Office of Science. Operation of the array at NSCL is supported by the NSF under Cooperative Agreement No. PHY-1102511 (NSCL) and DOE under Grant No. DE-AC02-05CH11231 (LBNL). B.A.B. acknowledges support from NSF Grant No. PHY-1068217. NR 31 TC 32 Z9 32 U1 0 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD OCT 16 PY 2013 VL 88 IS 4 AR 041302 DI 10.1103/PhysRevC.88.041302 PG 6 WC Physics, Nuclear SC Physics GA 240KT UT WOS:000326095500001 ER PT J AU Geballe, ZM Raju, SV Godwal, BK Jeanloz, R AF Geballe, Z. M. Raju, S. V. Godwal, B. K. Jeanloz, R. TI Clapeyron slope reversal in the melting curve of AuGa2 at 5.5 GPa SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article ID HIGH-PRESSURES; INTERMETALLIC COMPOUNDS; FLUORITE STRUCTURE; LIQUID; CALIBRATION; BEHAVIOR; ELEMENTS; SILICON; STATE AB We use x-ray diffraction in a resistively heated diamond anvil cell to extend the melting curve of AuGa2 beyond its minimum at 5.5 GPa and 720 K, and to constrain the high-temperature phase boundaries between cubic (fluorite structure), orthorhombic (cottunite structure) and monoclinic phases. We document a large change in Clapeyron slope that coincides with the transitions from cubic to lower symmetry phases, showing that a structural transition is the direct cause of the change in slope. In addition, moderate (similar to 30 K) to large (90 K) hysteresis is detected between melting and freezing, from which we infer that at high pressures, AuGa2 crystals can remain in a metastable state at more than 5% above the thermodynamic melting temperature. C1 [Geballe, Z. M.; Godwal, B. K.; Jeanloz, R.] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. [Raju, S. V.] Lawrence Berkeley Natl Lab, Berkeley, CA USA. RP Geballe, ZM (reprint author), Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. EM zgeballe@gmail.com FU National Science Foundation; COMPRES; ALS; Office of Science, Office of Basic Energy Sciences, of the US DoE [DE-AC02-05CH11231] FX Support for ZMG was provided by a National Science Foundation Graduate Research Fellowship. SVR thanks COMPRES and ALS for the financial support to carry out the above research work. The ALS is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the US DoE under Contract No. DE-AC02-05CH11231. NR 21 TC 1 Z9 1 U1 3 U2 13 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD OCT 16 PY 2013 VL 25 IS 41 AR 415401 DI 10.1088/0953-8984/25/41/415401 PG 7 WC Physics, Condensed Matter SC Physics GA 224VW UT WOS:000324920400008 PM 24025237 ER PT J AU Marney, LC Siegler, WC Parsons, BA Hoggard, JC Wright, BW Synovec, RE AF Marney, Luke C. Siegler, W. Christopher Parsons, Brendon A. Hoggard, Jamin C. Wright, Bob W. Synovec, Robert E. TI Tile-based Fisher-ratio software for improved feature selection analysis of comprehensive two-dimensional gas chromatography-time-of-flight mass spectrometry data SO TALANTA LA English DT Article DE Fisher ratio; Comprehensive two-dimensional gas chromatography; Time-of-flight mass spectrometry; Chemometrics; Feature selection ID GC X GC; CHEMOMETRIC ANALYSIS; ALIGNMENT ALGORITHM; TOFMS DATA; SEPARATIONS; ELIMINATION; MODULATION; INTERFACE; YEAST; FOOD AB Comprehensive two-dimensional (2D) gas chromatography coupled with time-of-flight mass spectrometry (GC x GC-TOFMS) is a highly capable instrumental platform that produces complex and information-rich multi-dimensional chemical data. The data can be initially overwhelming, especially when many samples (of various sample classes) are analyzed with multiple injections for each sample. Thus, the data must be analyzed in such a way as to extract the most meaningful information. The pixel-based and peak table-based Fisher ratio algorithmic approaches have been used successfully in the past to reduce the multi-dimensional data down to those chemical compounds that are changing between the sample classes relative to those that are not changing (i.e., chemical feature selection). We report on the initial development of a computationally fast novel tile-based Fisher-ratio software that addresses the challenges due to 2D retention time misalignment without explicitly aligning the data, which is often a shortcoming for both pixel-based and peak table-based algorithmic approaches. Concurrently, the tile-based Fisher-ratio algorithm significantly improves the sensitivity contrast of true positives against a background of potential false positives and noise. In this study, eight compounds, plus one internal standard, were spiked into diesel at various concentrations. The tile-based F-ratio algorithmic approach was able to "discover" all spiked analytes, within the complex diesel sample matrix with thousands of potential false positives, in each possible concentration comparison, even at the lowest absolute spiked analyte concentration ratio of 1.06, the ratio between the concentrations in the spiked diesel sample to the native concentration in diesel. (C) 2013 Elsevier B.V. All rights reserved. C1 [Marney, Luke C.; Siegler, W. Christopher; Parsons, Brendon A.; Hoggard, Jamin C.; Synovec, Robert E.] Univ Washington, Dept Chem, Seattle, WA 98198 USA. [Wright, Bob W.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Synovec, RE (reprint author), Univ Washington, Dept Chem, POB 351700, Seattle, WA 98198 USA. EM synovec@chem.washington.edu OI Parsons, Brendon/0000-0002-4411-0063 FU Internal Revenue Service (IRS); US Department of Energy (DOE) [DE-AC05-76RLO 1830]; Pacific Northwest National Laboratory FX This work was supported by the Internal Revenue Service (IRS) under an Interagency Agreement with the US Department of Energy (DOE) under Contract DE-AC05-76RLO 1830 with the Pacific Northwest National Laboratory. Battelle Memorial Institute operates the Pacific Northwest National Laboratory. NR 30 TC 13 Z9 13 U1 0 U2 22 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0039-9140 EI 1873-3573 J9 TALANTA JI Talanta PD OCT 15 PY 2013 VL 115 BP 887 EP 895 DI 10.1016/j.talanta.2013.06.038 PG 9 WC Chemistry, Analytical SC Chemistry GA 267KD UT WOS:000328095600127 PM 24054679 ER PT J AU Harding, LB Schultz, IR Goetz, GW Luckenbach, JA Young, G Goetz, FW Swanson, P AF Harding, Louisa B. Schultz, Irvin R. Goetz, Giles W. Luckenbach, J. Adam Young, Graham Goetz, Frederick W. Swanson, Penny TI High-throughput sequencing and pathway analysis reveal alteration of the pituitary transcriptome by 17 alpha-ethynylestradiol (EE2) in female coho salmon, Oncorhynchus kisutch SO AQUATIC TOXICOLOGY LA English DT Article DE Endocrine disruption; Fish reproduction; Pituitary; Gonadotropins; Circadian rhythm; Transcriptomics ID ZEBRAFISH DANIO-RERIO; FOLLICLE-STIMULATING-HORMONE; MINNOWS PIMEPHALES-PROMELAS; ENVIRONMENTAL ENDOCRINE DISRUPTERS; DIFFERENTIAL EXPRESSION ANALYSIS; GRAPHICAL SYSTEMS-MODEL; BETA-SUBUNIT GENE; GROWTH-FACTOR-I; RNA-SEQ DATA; RAINBOW-TROUT AB Considerable research has been done on the effects of endocrine disrupting chemicals (EDCs) on reproduction and gene expression in the brain, liver and gonads of teleost fish, but information on impacts to the pituitary gland are still limited despite its central role in regulating reproduction. The aim of this study was to further our understanding of the potential effects of natural and synthetic estrogens on the brain-pituitary-gonad axis in fish by determining the effects of 17 alpha-ethynylestradiol (EE2) on the pituitary transcriptome. We exposed sub-adult coho salmon (Oncorhynchus kisutch) to 0 or 12 ng EE2/L for up to 6 weeks and effects on the pituitary transcriptome of females were assessed using high-throughput Illumina (R) sequencing, RNA-Seq and pathway analysis. After 1 or 6 weeks, 218 and 670 contiguous sequences (contigs) respectively, were differentially expressed in pituitaries of EE2-exposed fish relative to control. Two of the most highly up- and down-regulated contigs were luteinizing hormone beta subunit (241-fold and 395-fold at 1 and 6 weeks, respectively) and follicle-stimulating hormone beta subunit (-3.4-fold at 6 weeks). Additional contigs related to gonadotropin synthesis and release were differentially expressed in EE2-exposed fish relative to controls. These included contigs involved in gonadotropin releasing hormone (GNRH) and transforming growth factor-beta signaling. There was an over-representation of significantly affected contigs in 33 and 18 canonical pathways at 1 and 6 weeks, respectively, including circadian rhythm signaling, calcium signaling, peroxisome proliferator-activated receptor (PPAR) signaling, PPAR alpha/retinoid x receptor alpha activation, and netrin signaling. Network analysis identified potential interactions between genes involved in circadian rhythm and GNRH signaling, suggesting possible effects of EE2 on timing of reproductive events. Published by Elsevier B.V. C1 [Harding, Louisa B.; Goetz, Giles W.; Young, Graham] Univ Washington, Sch Aquat & Fishery Sci, Seattle, WA 98195 USA. [Schultz, Irvin R.] Pacific NW Natl Lab, Marine Sci Lab, Battelle, Sequim, WA 98382 USA. [Luckenbach, J. Adam; Swanson, Penny] Natl Ocean & Atmospher Adm, NW Fisheries Sci Ctr, Natl Marine Fisheries Serv, Seattle, WA 98112 USA. [Luckenbach, J. Adam; Young, Graham; Swanson, Penny] Washington State Univ, Ctr Reprod Biol, Pullman, WA 98164 USA. [Goetz, Frederick W.] Natl Ocean & Atmospher Adm, NW Fisheries Sci Ctr, Natl Marine Fisheries Serv, Manchester Res Stn, Manchester, WA 98353 USA. RP Swanson, P (reprint author), Natl Ocean & Atmospher Adm, NW Fisheries Sci Ctr, Natl Marine Fisheries Serv, 2725 Montlake Blvd E, Seattle, WA 98112 USA. EM penny.swanson@noaa.gov FU Washington Sea Grant Project [RB-49]; Richard T. Whiteleather scholarship; Melvin Anderson Endowed Scholarship in Fisheries; Roy Jensen Research Fellowship; Lauren R. Donaldson Scholarship FX Funding for this project was provided by Washington Sea Grant Project RB-49 and scholarships to Louisa Harding from the Richard T. Whiteleather scholarship, the Melvin Anderson Endowed Scholarship in Fisheries, the Roy Jensen Research Fellowship, and the Lauren R. Donaldson Scholarship. The authors also wish to acknowledge Abby Tillotson, Jon Dickey, and Mollie Middleton for technical assistance with fish sampling and Dr. Josep Planas for valuable comments during the drafting of this manuscript. NR 107 TC 13 Z9 14 U1 7 U2 60 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0166-445X EI 1879-1514 J9 AQUAT TOXICOL JI Aquat. Toxicol. PD OCT 15 PY 2013 VL 142 BP 146 EP 163 DI 10.1016/j.aquatox.2013.07.020 PG 18 WC Marine & Freshwater Biology; Toxicology SC Marine & Freshwater Biology; Toxicology GA 267JM UT WOS:000328093900015 PM 24007788 ER PT J AU Fox, BP Simmons-Potter, K Kliner, DAV Moore, SW AF Fox, Brian P. Simmons-Potter, Kelly Kliner, Dahv A. V. Moore, Sean W. TI Effect of low-earth orbit space on radiation-induced absorption in rare-earth-doped optical fibers SO JOURNAL OF NON-CRYSTALLINE SOLIDS LA English DT Article DE Rare-earth; Optical fiber; Space radiation; Color-center; Ionizing-radiation effects ID COLOR-CENTERS; SILICA FIBERS; SMOKY QUARTZ; HIGH-POWER; DOSE-RATE; GAMMA; YTTERBIUM; LUMINESCENCE; ATTENUATION; GLASSES AB The implementation of optical systems, based on rare-earth doped fibers, in space environments adds a powerful new dimension of functionality to the design of space-based systems, particularly when high power and bandwidth, high fidelity, and low susceptibility to electromagnetic interference are desired. As these specialty fibers are often the most sensitive components of an optical system, extensive use requires considerable insight into the ionizing-radiation-induced changes experienced by the fibers during their operational lifetime. In this research, a suite of aluminosilicate fibers singly or co-doped with erbium and ytterbium ions was deployed into low-Earth orbit for approximately 18 months as part of the Materials International Space Station Experiment (MISSE) 7 mission. Optical spectroscopy performed on the retrieved fibers is compared to control data from pristine, unirradiated fibers, revealing colorcenter generation in the visible portion of the spectrum consistent with silica-related and aluminum-related absorption centers, with band-tailing into the near-infrared. Results suggest that visible to near infra-red (NIR) absorption experienced by the co-doped fiber is less-pronounced than in its singly-doped counterparts, likely a result of the lower aluminum concentration of this fiber. The data were also compared to data from terrestrial Co-60 irradiation of the same fiber types and it was found that the overall trends observed in the space-irradiated fibers in the near-infrared were accurately, although not identically, reproduced. The resultant information is important for the design and testing of radiation-hardened optical-fiber-based laser and amplifier systems. (C) 2013 Elsevier B.V. All rights reserved. C1 [Fox, Brian P.; Simmons-Potter, Kelly] Univ Arizona, Tucson, AZ 85721 USA. [Kliner, Dahv A. V.] nLight, Vancouver, WA 98665 USA. [Moore, Sean W.] Sandia Natl Labs, Livermore, CA 94551 USA. RP Fox, BP (reprint author), Univ Arizona, Tucson, AZ 85721 USA. EM bpf@email.arizona.edu RI shao, chongyun/M-6620-2013 FU University of Arizona, State of Arizona TRIF [301]; United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was primarily supported by the University of Arizona, State of Arizona TRIF funds under Proposition 301 and secondarily supported by Sandia National Laboratories. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy's National Nuclear Security Administration, under contract DE-AC04-94AL85000. The authors are indebted to Gayle Thayer of Sandia National Laboratories and to Phil Jenkins and Kelly M. Trautz of the Naval Research Laboratories for their help with the MISSE-7 integration portion of the research. NR 43 TC 5 Z9 5 U1 6 U2 27 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3093 EI 1873-4812 J9 J NON-CRYST SOLIDS JI J. Non-Cryst. Solids PD OCT 15 PY 2013 VL 378 BP 79 EP 88 DI 10.1016/j.jnoncrysol.2013.06.009 PG 10 WC Materials Science, Ceramics; Materials Science, Multidisciplinary SC Materials Science GA 255ZR UT WOS:000327279800012 ER PT J AU Kerisit, S Ryan, JV Pierce, EM AF Kerisit, Sebastien Ryan, Joseph V. Pierce, Eric M. TI Monte Carlo simulations of the corrosion of aluminoborosilicate glasses SO JOURNAL OF NON-CRYSTALLINE SOLIDS LA English DT Article DE Aluminoborosilicate glasses; Glass corrosion; Monte Carlo simulations ID NUCLEAR-WASTE GLASSES; FLOW-THROUGH EXPERIMENTS; BOROSILICATE GLASSES; DISSOLUTION RATES; EQUILIBRIUM CONDITIONS; AQUEOUS ALTERATION; ALKALINE MEDIA; RATE LAW; GEL; SURFACE AB Aluminum is one of the most common components included in nuclear waste glasses. Therefore, Monte Carlo (MC) simulations were carried out to investigate the influence of aluminum on the rate and mechanism of dissolution of sodium borosilicate glasses in static conditions. The glasses studied were in the compositional range (70 - 2x)% SiO2 x% Al2O3 15% B2O3 (15 + x)% Na2O, where 0 <= x <= 15%. The simulation results show that increasing amounts of aluminum in the pristine glasses slow down the initial rate of dissolution as determined from the rate of boron release. However, the extent of corrosion - as measured by the total amount of boron release - initially increases with addition of Al2O3, up to 5 mol% Al2O3, but subsequently decreases with further Al2O3 addition. The MC simulations reveal that this behavior is due to the interplay between two opposing mechanisms: (1) aluminum slows down the kinetics of hydrolysis/condensation reactions that drive the reorganization of the glass surface and eventual formation of a blocking layer; and (2) aluminum strengthens the glass thereby increasing the lifetime of the upper part of its surface and allowing for more rapid formation of a blocking layer. Additional MC simulations were performed whereby a process representing the formation of a secondary aluminosilicate phase was included. Secondary phase formation draws dissolved glass components out of the aqueous solution, thereby diminishing the rate of condensation and delaying the formation of a blocking layer. As a result, the extent of corrosion is found to increase continuously with increasing Al2O3 content, as observed experimentally. For Al2O3 < 10 mol%, the MC simulations also indicate that, because the secondary phase solubility eventually controls the aluminum content in the part of the altered layer in contact with the bulk aqueous solution, the dissolved aluminum and silicon concentrations at steady state are not dependent on the Al2O3 content of the pristine aluminoborosilicate glass. (C) 2013 Elsevier B.V. All rights reserved. C1 [Kerisit, Sebastien] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. [Ryan, Joseph V.] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. [Pierce, Eric M.] Oak Ridge Natl Lab, Energy & Environm Sci Directorate, Oak Ridge, TN 37831 USA. RP Kerisit, S (reprint author), Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. EM sebastien.kerisit@pnnl.gov RI Pierce, Eric/G-1615-2011 OI Pierce, Eric/0000-0002-4951-1931 FU U.S. Department of Energy's Office of Nuclear Energy (Fuel Cycle Research and Development); Office of Environmental Management (Tank Waste Mgmt) [EM-21]; Office of Science's Office of Biological and Environmental Research (OBER); DOE by Battelle Memorial Institute [DE-ACO5-76RL01830]; DOE [DE-AC05-000R22725] FX This work was jointly funded by the U.S. Department of Energy's Office of Nuclear Energy (Fuel Cycle Research and Development) and the Office of Environmental Management (Tank Waste Mgmt, EM-21). Some computer simulations were performed as part of a DOE Office of Science-supported Science Theme User Proposal at the William R. Wiley Environmental Molecular Sciences Laboratory (EMSL) Molecular Science Computing (MSC) facilities. The EMSL is a national scientific user facility sponsored by the Office of Science's Office of Biological and Environmental Research (OBER) and located at the Pacific Northwest National Laboratory (PNNL). PNNL is operated for the DOE by Battelle Memorial Institute under Contract DE-ACO5-76RL01830. Oak Ridge National Laboratory (ORNL) is managed by UT-Battelle LLC for the DOE under contract DE-AC05-000R22725. NR 49 TC 8 Z9 9 U1 7 U2 27 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3093 EI 1873-4812 J9 J NON-CRYST SOLIDS JI J. Non-Cryst. Solids PD OCT 15 PY 2013 VL 378 BP 273 EP 281 DI 10.1016/j.jnoncrysol.2013.07.014 PG 9 WC Materials Science, Ceramics; Materials Science, Multidisciplinary SC Materials Science GA 255ZR UT WOS:000327279800041 ER PT J AU Olsen, BN Bielska, AA Lee, T Daily, MD Covey, DF Schlesinger, PH Baker, NA Ory, DS AF Olsen, Brett N. Bielska, Agata A. Lee, Tiffany Daily, Michael D. Covey, Douglas F. Schlesinger, Paul H. Baker, Nathan A. Ory, Daniel S. TI The Structural Basis of Cholesterol Accessibility in Membranes SO BIOPHYSICAL JOURNAL LA English DT Article ID MOLECULAR-DYNAMICS SIMULATIONS; CONDENSED COMPLEXES; LIPID-BILAYERS; PHOSPHOLIPIDS; HOMEOSTASIS; CELL; DIPALMITOYLPHOSPHATIDYLCHOLINE; ACTIVATION; PATHWAY AB Although the majority of free cellular cholesterol is present in the plasma membrane, cholesterol homeostasis is principally regulated through sterol-sensing proteins that reside in the cholesterol-poor endoplasnnic reticulum (ER). In response to acute cholesterol loading or depletion, there is rapid equilibration between the ER and plasma membrane cholesterol pools, suggesting a biophysical model in which the availability of plasma membrane cholesterol for trafficking to internal membranes modulates ER membrane behavior. Previous studies have predominantly examined cholesterol availability in terms of binding to extrannembrane acceptors, but have provided limited insight into the structural changes underlying cholesterol activation. In this study, we use both molecular dynamics simulations and experimental membrane systems to examine the behavior of cholesterol in membrane bilayers. We find that cholesterol depth within the bilayer provides a reasonable structural metric for cholesterol availability and that this is correlated with cholesterol-acceptor binding. Further, the distribution of cholesterol availability in our simulations is continuous rather than divided into distinct available and unavailable pools. This data provide support for a revised cholesterol activation model in which activation is driven not by saturation of membrane-cholesterol interactions but rather by bulk membrane remodeling that reduces membrane-cholesterol affinity. C1 [Olsen, Brett N.; Bielska, Agata A.; Lee, Tiffany; Ory, Daniel S.] Washington Univ, Sch Med, Diabet Cardiovasc Dis Ctr, St Louis, MO 63130 USA. [Daily, Michael D.; Baker, Nathan A.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Covey, Douglas F.] Washington Univ, Sch Med, Dept Dev Biol, St Louis, MO USA. [Schlesinger, Paul H.] Washington Univ, Sch Med, Dept Cell Biol & Physiol, St Louis, MO 63110 USA. RP Ory, DS (reprint author), Washington Univ, Sch Med, Diabet Cardiovasc Dis Ctr, St Louis, MO 63130 USA. EM dory@dom.wustl.edu RI Baker, Nathan/A-8605-2010 OI Baker, Nathan/0000-0002-5892-6506 FU National Institutes of Health [R01 HL067773]; Institutional Cardiovascular Biology Training [T32111-007275]; National Institutes of Health (NIH) [F30 HL97563]; National Biorhedical Computation Resource [NM P41 RR0860516]; Extreme Science and Engineering Discovery Environment (XSEDE); National Science Foundation [OCI1053575]; [TG-MCB060053]; [TG-MCAO8X003] FX This work was supported by the National Institutes of Health through grant No. R01 HL067773. B.N.O. was supported by the Institutional Cardiovascular Biology Training Grant, grant No. T32111-007275. A.A.G. was supported by the National Institutes of Health (NIH) through grant No. F30 HL97563. Computational resources were provided by the Texas Advanced Computing Center through Teragrid grants No. TG-MCB060053 and TG-MCAO8X003 as well as the National Biorhedical Computation Resource through grant No. NM P41 RR0860516. This work used the Extreme Science and Engineering Discovery Environment (XSEDE), which is supported by the National Science Foundation through grant No. OCI1053575. NR 49 TC 13 Z9 13 U1 1 U2 23 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD OCT 15 PY 2013 VL 105 IS 8 BP 1838 EP 1847 DI 10.1016/j.bpj.2013.08.042 PG 10 WC Biophysics SC Biophysics GA 236ZR UT WOS:000325838500014 PM 24138860 ER PT J AU Guildenbecher, DR Reu, PL Stuaffacher, HL Grasser, T AF Guildenbecher, Daniel R. Reu, Phillip L. Stuaffacher, Howard Lee Grasser, Thomas TI Accurate measurement of out-of-plane particle displacement from the cross correlation of sequential digital in-line holograms SO OPTICS LETTERS LA English DT Article ID POSITION AB A new method to quantify three-dimensional particle fields using digital in-line holography is presented. From sequentially recorded holograms, the maximum cross correlation of edge sharpness within local particle windows yields an accurate measurement of particle displacements. Experiments demonstrate out-of-plane displacement uncertainty of approximately 0.15 mean particle diameters, which is roughly an order-of-magnitude improvement compared with alternative methods. Application to shotgun pellets demonstrates robustness despite experimental noise. (C) 2013 Optical Society of America C1 [Guildenbecher, Daniel R.; Reu, Phillip L.; Stuaffacher, Howard Lee; Grasser, Thomas] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Guildenbecher, DR (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM drguild@sandia.gov FU United States Department of Energy's National Nuclear Security Administration [DEAC04-94AL85000] FX Sandia National Laboratories is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy's National Nuclear Security Administration under contract no. DEAC04-94AL85000. NR 10 TC 7 Z9 7 U1 1 U2 6 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 0146-9592 EI 1539-4794 J9 OPT LETT JI Opt. Lett. PD OCT 15 PY 2013 VL 38 IS 20 BP 4015 EP 4018 DI 10.1364/OL.38.004015 PG 4 WC Optics SC Optics GA 246WD UT WOS:000326570300011 PM 24321909 ER PT J AU van Tilborg, J Shaw, BH Sokollik, T Rykovanov, S Monchoce, S Quere, F Martin, P Malvache, A Leemans, WP AF van Tilborg, J. Shaw, B. H. Sokollik, T. Rykovanov, S. Monchoce, S. Quere, F. Martin, Ph. Malvache, A. Leemans, W. P. TI Spectral characterization of laser-driven solid-based high harmonics in the coherent wake emission regime SO OPTICS LETTERS LA English DT Article ID PLASMA SURFACES; GENERATION; ABSORPTION; PULSE AB Laser-produced surface high-harmonic generation is an attractive source of extreme ultraviolet radiation due to its coherent properties and high peak power. By operating at subrelativistic laser intensities in the coherent wake emission regime, the harmonic spectrum was experimentally studied versus laser properties. At higher laser intensities (>10(17) W/cm(2)) a higher spectral cutoff was observed, with accompanying blueshifting and spectral broadening of the individual orders. A model based on an expanding critical surface provides qualitative agreement with the observations. (C) 2013 Optical Society of America C1 [van Tilborg, J.; Shaw, B. H.; Sokollik, T.; Rykovanov, S.; Leemans, W. P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Monchoce, S.; Quere, F.; Martin, Ph.] CEA, IRAMIS, Serv Photons Atomes & Mol, F-91191 Gif Sur Yvette, France. [Malvache, A.] Ecole Polytech, Lab Opt Appl, ENSTA ParisTech, CNRS,UMR 7639, F-91761 Palaiseau, France. RP van Tilborg, J (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM JvanTilborg@lbl.gov RI Quere, Fabien/F-2638-2014; Sokollik, Thomas/P-2584-2015; Malvache, Arnaud/O-4082-2016 OI Malvache, Arnaud/0000-0002-0792-3460 FU Office of Science, Office of High Energy Physics, of the U.S. Department of Energy [DE-AC02-05CH11231]; France-Berkeley fund FX This work was supported by the director, Office of Science, Office of High Energy Physics, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231, as well as the France-Berkeley fund. NR 20 TC 5 Z9 5 U1 1 U2 15 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 0146-9592 EI 1539-4794 J9 OPT LETT JI Opt. Lett. PD OCT 15 PY 2013 VL 38 IS 20 BP 4026 EP 4029 DI 10.1364/OL.38.004026 PG 4 WC Optics SC Optics GA 246WD UT WOS:000326570300014 PM 24321912 ER PT J AU Rubenchik, AM Tkachenko, EV Fedoruk, MP Turitsyn, SK AF Rubenchik, A. M. Tkachenko, E. V. Fedoruk, M. P. Turitsyn, S. K. TI Power-controlled phase-matching and instability of CW propagation in multicore optical fibers with a central core SO OPTICS LETTERS LA English DT Article ID WAVE-GUIDE ARRAYS; MODULATION INSTABILITY; DISCRETE SOLITONS; LOCALIZED MODES; DYNAMICS; SYSTEMS AB We present modulation instability analysis including azimuthal perturbations of steady-state continuous wave (CW) propagation in multicore-fiber configurations with a central core. In systems with a central core, a steady CW evolution regime requires power-controlled phase matching, which offers interesting spatial-division applications. Our results have general applicability and are relevant to a range of physical and engineering systems, including high-power fiber lasers, optical transmission in multicore fiber, and systems of coupled nonlinear waveguides. (C) 2013 Optical Society of America C1 [Rubenchik, A. M.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Tkachenko, E. V.; Fedoruk, M. P.] SB RAS, Inst Computat Technol, Novosibirsk 630090, Russia. [Fedoruk, M. P.; Turitsyn, S. K.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Turitsyn, S. K.] Aston Univ, Aston Inst Photon Technol, Birmingham B4 7ET, W Midlands, England. RP Turitsyn, SK (reprint author), Novosibirsk State Univ, Novosibirsk 630090, Russia. EM s.k.turitsyn@aston.ac.uk RI Turitsyn, Sergei/J-5562-2013 OI Turitsyn, Sergei/0000-0003-0101-3834 FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; EPSRC [EP/J017582/1]; Ministry of Education and Science of the Russian Federation [14.B25.31.0003]; European Research Council (UL-TRALASER); Marie Curie IRSES FX This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. The financial support of the EPSRC program grant UN-LOC (EP/J017582/1), grant of the Ministry of Education and Science of the Russian Federation (agreement no. 14.B25.31.0003), the European Research Council (UL-TRALASER) and the Marie Curie IRSES program is acknowledged. NR 23 TC 11 Z9 11 U1 1 U2 17 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 0146-9592 EI 1539-4794 J9 OPT LETT JI Opt. Lett. PD OCT 15 PY 2013 VL 38 IS 20 BP 4232 EP 4235 DI 10.1364/OL.38.004232 PG 4 WC Optics SC Optics GA 246WD UT WOS:000326570300069 PM 24321967 ER PT J AU Roccaro, P Chang, HS Vagliasindi, FGA Korshin, GV AF Roccaro, Paolo Chang, Hyun-shik Vagliasindi, Federico G. A. Korshin, Gregory V. TI Modeling bromide effects on yields and speciation of dihaloacetonitriles formed in chlorinated drinking water SO WATER RESEARCH LA English DT Article DE Nitrogenous disinfection by-products; Natural organic matter; Chlorine dose; Reaction time; Temperature; pH ID DISINFECTION BY-PRODUCTS; DISSOLVED ORGANIC-MATTER; COLLECTION RULE DATABASE; DIFFERENTIAL ABSORBENCY; TRIHALOMETHANE FORMATION; THM FORMATION; NITROGEN; DBPS; CHLORAMINATION; HALOACETONITRILES AB This study examined effects of bromide on yields and speciation of dihaloacetonitrile (DHAN) species that included dichloro-, bromochloro- and dibromoacetonitriles generated in chlorinated water. Experimental data obtained using two water sources, varying concentrations and characters of Natural Organic Matter (NOM), bromide concentrations, reaction times, chlorine doses, temperatures and pHs were interpreted using a semi-phenomenological model that assumed the presence of three kinetically distinct sites in NOM (denoted as sites S-1, S-2 and S-3) and the occurrence of sequential incorporation of bromine and chlorine into them. One site was found to react very fast with the chlorine and bromine but its contribution in the DHAN generation was very low. The site with the highest contribution to the yield of DHAN (>70%) has the lowest reaction rates. The model introduced dimensionless coefficients (denoted as phi(DHAN)(1), phi(DHAN)(2) and phi(DHAN)(3)) applicable to the initial DHAN generation sites and their monochlorinated and monobrominated products, respectively. These parameters were used to quantify the kinetic preference to bromine incorporation over that of chlorine. Values of these coefficients optimized for DHAN formation were indicative of the strongly preferential incorporation of bromine into the engaged NOM sites. The same set of phi(DHAN)(i) coefficients could be used to model the speciation of DHAN released from their kinetically different precursors. The dimensionless speciation coefficients phi(DHAN)(i) were determined to be site specific and dependent on the NOM content and character as well as pH. The presented model of DHAN formation and speciation can help quantify in more detail the generation of DHAN and provide more insight necessary for further assessment of their potential health effects. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Roccaro, Paolo; Vagliasindi, Federico G. A.] Univ Catania, Dept Civil & Environm Engn, I-95124 Catania, Italy. [Chang, Hyun-shik] Savannah River Ecol Lab, Aiken, SC 29802 USA. [Korshin, Gregory V.] Univ Washington, Dept Civil & Environm Engn, Seattle, WA 98195 USA. RP Roccaro, P (reprint author), Univ Catania, Dept Civil & Environm Engn, I-95124 Catania, Italy. EM proccaro@dica.unict.it RI Roccaro, Paolo/B-2432-2015; OI Roccaro, Paolo/0000-0002-5504-8082; VAGLIASINDI, FEDERICO G. A./0000-0002-9648-4171; Korshin, Gregory/0000-0002-9226-6601 FU United States EPA/Cadmus [069-UW-1]; Italian Ministry of Instruction, University, and Research (MIUR); US-Italy Fulbright Commission; Australian International Center of Excellence in Water Resources Management (ICE WaRM); Department of Energy [DEFC09-07-SR22506]; University of Georgia research Foundation [DEFC09-07-SR22506] FX This study was partially supported by the United States EPA/Cadmus (grant 069-UW-1), and the Italian Ministry of Instruction, University, and Research (MIUR), through the Research Projects of National Interest "Control and Monitoring of Drinking Water Quality" and "Reuse of Wastewater in Agriculture: Emerging Pollutants and Operational Problems". Views expressed in this paper do not necessarily reflect those of the funding agencies. Paolo Roccaro acknowledges the US-Italy Fulbright Commission for supporting his research in the US through the "Fulbright Scholar Program Advanced Research and University Lecturing Awards in the United States". Gregory Korshin acknowledges support from the Australian International Center of Excellence in Water Resources Management (ICE WaRM) that contributed to his work on the concepts presented in this paper. Hyun-shik Chang acknowledges the support of a cooperative agreement (DEFC09-07-SR22506) between the Department of Energy and the University of Georgia research Foundation. The authors also thank Prof. Mark Benjamin for his valuable suggestions concerning this study. NR 48 TC 14 Z9 14 U1 5 U2 53 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0043-1354 J9 WATER RES JI Water Res. PD OCT 15 PY 2013 VL 47 IS 16 BP 5995 EP 6006 DI 10.1016/j.watres.2013.07.018 PG 12 WC Engineering, Environmental; Environmental Sciences; Water Resources SC Engineering; Environmental Sciences & Ecology; Water Resources GA 251EG UT WOS:000326910000004 PM 24035655 ER PT J AU Evans, AM Wright, JM Meyer, A Rivera-Nunez, Z AF Evans, Amanda M. Wright, J. Michael Meyer, Amy Rivera-Nunez, Zorimar TI Spatial variation of disinfection by-product concentrations: Exposure assessment implications SO WATER RESEARCH LA English DT Article DE Exposure misclassification; Bias; Exposure measurement error; Brominated trihalomethanes; Haloacetic acids; Environmental epidemiology; Intra-system variability ID FOR-GESTATIONAL-AGE; WATER DISTRIBUTION-SYSTEM; DRINKING-WATER; BIRTH-WEIGHT; TRIHALOMETHANE EXPOSURE; SPONTANEOUS-ABORTION; FETAL-GROWTH; TAP WATER; VARIABILITY; PREGNANCY AB The use of public water system (PWS) average trihalomethane (THM) and haloacetic acid (HAA) concentrations as surrogates of "personal" exposures in epidemiological studies of disinfection by-products (DBPs) may result in exposure misclassification bias from various sources of measurement error including intra-system variation of DBPs. Using 2000-2004 data from 107 PWSs in Massachusetts, we assessed two approaches for characterizing DBP spatial variability by identifying PWSs with low spatial variability (LSV) and examining differences in LSV across DBP groups and by type of source water and primary disinfectant. We also used spatial differences to examine the association between THM concentrations and indices of social disadvantage; however, we found no correlations or statistically significant differences based on the available data. We observed similar patterns for the percentage of quarterly sampling dates with LSV across different types of source water for all DBPs but not across disinfectants. We found there was little overlap between sites classified as having LSV across different DBP groups. In the main analysis, we found moderate correlations between both approaches (phi(THM4) = 0.55; phi(BrTHM) = 0.64; phi(HAA5) = 0.67); although Method 1 (based on concentration differences between samples) may be better - suited for identifying PWSs for inclusion in epidemiological studies because it is more easily adapted to study-specific exposure gradients than Method 2 (based on categorical exposure percentiles). These data reinforce the need to consider different exposure assessment approaches when examining the spatial variation of multiple DBP surrogates as they can represent different DBP mixtures. (C)n2013 Elsevier Ltd. All rights reserved. C1 [Evans, Amanda M.; Meyer, Amy] Oak Ridge Inst Sci & Educ, Cincinnati, OH 45268 USA. [Wright, J. Michael] US EPA, Natl Ctr Environm Assessment, Off Res & Dev, Cincinnati, OH 45268 USA. [Rivera-Nunez, Zorimar] CNR, Cincinnati, OH 45268 USA. RP Evans, AM (reprint author), Oak Ridge Inst Sci & Educ, 26 West Martin Luther King Blvd MS-A110, Cincinnati, OH 45268 USA. EM evans.amandam@epa.gov; wright.michael@epa.gov; meyer-anxu@gmail.com; znunez@wustl.edu FU Research Participation Program at the National Center for Environmental Assessment, Office of Research and Development, U.S. Environmental Protection Agency (EPA) FX The authors would like to thank the Massachusetts Department of Environmental Protection offices, the Massachusetts Water Resource Authority, and other public water utilities for their assistance with the data collection efforts. This project was supported in part by an appointment to the Research Participation Program at the National Center for Environmental Assessment, Office of Research and Development, U.S. Environmental Protection Agency (EPA), administered by the Oak Ridge Institute for Science and Education through an interagency agreement between the U.S. Department of Energy and EPA. The views expressed herein are those of the authors and do not necessarily reflect the views or policies of the EPA. NR 56 TC 6 Z9 6 U1 0 U2 40 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0043-1354 J9 WATER RES JI Water Res. PD OCT 15 PY 2013 VL 47 IS 16 BP 6130 EP 6140 DI 10.1016/j.watres.2013.07.032 PG 11 WC Engineering, Environmental; Environmental Sciences; Water Resources SC Engineering; Environmental Sciences & Ecology; Water Resources GA 251EG UT WOS:000326910000017 PM 23993731 ER PT J AU Zhang, Y Xie, JP Liu, MM Tian, Z He, ZL van Nostrand, JD Ren, LR Zhou, JZ Yang, M AF Zhang, Yu Xie, Jianping Liu, Miaomiao Tian, Zhe He, Zhili van Nostrand, Joy D. Ren, Liren Zhou, Jizhong Yang, Min TI Microbial community functional structure in response to antibiotics in pharmaceutical wastewater treatment systems SO WATER RESEARCH LA English DT Article DE Antibiotic production wastewater; Antibiotic resistance; Fungi; Geochip ID TETRACYCLINE RESISTANCE GENES; GEOCHIP-BASED ANALYSIS; ACTIVATED-SLUDGE; RECEIVING RIVER; POPULATION-DYNAMICS; TREATMENT-PLANT; PENICILLIN-G; DIVERSITY; BACTERIA; OIL AB It is widely demonstrated that antibiotics in the environment affect microbial community structure. However, direct evidence regarding the impacts of antibiotics on microbial functional structures in wastewater treatment systems is limited. Herein, a high-throughput functional gene array (GeoChip 3.0) in combination with quantitative PCR and clone libraries were used to evaluate the microbial functional structures in two biological wastewater treatment systems, which treat antibiotic production wastewater mainly containing oxytetracycline. Despite the bacteriostatic effects of antibiotics, the GeoChip detected almost all key functional gene categories, including carbon cycling, nitrogen cycling, etc., suggesting that these microbial communities were functionally diverse. Totally 749 carbon-degrading genes belonging to 40 groups (24 from bacteria and 16 from fungi) were detected. The abundance of several fungal carbon-degrading genes (e.g., glyoxal oxidase ( glx), lignin peroxidase or ligninase (lip), manganese peroxidase (mnp), endochitinase, exoglucanase_genes) was significantly correlated with antibiotic concentrations (Mantel teSt; P < 0.05), showing that the fungal functional genes have been enhanced by the presence of antibiotics. However, from the fact that the majority of carbon-degrading genes were derived from bacteria and diverse antibiotic resistance genes were detected in bacteria, it was assumed that many bacteria could survive in the environment by acquiring antibiotic resistance and may have maintained the position as a main player in nutrient removal. Variance partitioning analysis showed that antibiotics could explain 24.4% of variations in microbial functional structure of the treatment systems. This study provides insights into the impacts of antibiotics on microbial functional structure of a unique system receiving antibiotic production wastewater, and reveals the potential importance of the cooperation between fungi and bacteria with antibiotic resistance in maintaining the stability and performance of the systems. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Zhang, Yu; Liu, Miaomiao; Tian, Zhe; Yang, Min] Chinese Acad Sci, Res Ctr Ecoenvironm Sci, State Key Lab Environm Aquat Chem, Beijing 100085, Peoples R China. [Xie, Jianping; He, Zhili; van Nostrand, Joy D.; Zhou, Jizhong] Univ Oklahoma, Inst Environm Genom, Dept Microbiol & Plant Biol, Norman, OK 73019 USA. [Xie, Jianping] Cent S Univ, Sch Mineral Proc & Bioengn, Changsha 410083, Hunan, Peoples R China. [Ren, Liren] North China Pharmaceut Grp Corp, Inst Environm Sci & Technol, Shijiazhuang, Hebei, Peoples R China. [Zhou, Jizhong] Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94270 USA. [Zhou, Jizhong] Tsinghua Univ, Sch Environm, State Key Joint Lab Environm Simulat & Pollut Con, Beijing 100084, Peoples R China. RP Yang, M (reprint author), 18 Shuangqing Rd, Beijing 100085, Peoples R China. EM yangmin@rcees.ac.cn RI Van Nostrand, Joy/F-1740-2016 OI Van Nostrand, Joy/0000-0001-9548-6450 FU National Natural Scientific Foundation of China (NSFC) [51178449, 21277162, 51221892]; special fund of State key Joint Laboratory of Environment Simulation and Pollution Control [12L03ESPC]; ENIGMA - Ecosystems and Networks Integrated with Genes and Molecular Assemblies through the Office of Science, Office of Biological and Environmental Research; U. S. Department of Energy [DE-ACO2-05CH11231] FX This study was supported by National Natural Scientific Foundation of China (NSFC: 51178449; 21277162, 51221892) and by special fund of State key Joint Laboratory of Environment Simulation and Pollution Control (12L03ESPC). This study made use of the Geo Chip and associated computational pipelines whose development was funded by ENIGMA - Ecosystems and Networks Integrated with Genes and Molecular Assemblies through the Office of Science, Office of Biological and Environmental Research, the U. S. Department of Energy under Contract No. DE-ACO2-05CH11231. We thank Dr. Yunfeng Yang, Dr. Yuting Liang and Dr. Hongwei Zhou for their help in statistical analysis and manuscript revising. NR 50 TC 16 Z9 21 U1 16 U2 201 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0043-1354 J9 WATER RES JI Water Res. PD OCT 15 PY 2013 VL 47 IS 16 BP 6298 EP 6308 DI 10.1016/j.watres.2013.08.003 PG 11 WC Engineering, Environmental; Environmental Sciences; Water Resources SC Engineering; Environmental Sciences & Ecology; Water Resources GA 251EG UT WOS:000326910000032 PM 23981791 ER PT J AU Shah, V Shah, S Mackey, H Kambhampati, M Collins, D Dowd, SE Colichio, R McDonnell, KT Green, T AF Shah, Vishal Shah, Shreya Mackey, Herman Kambhampati, Murty Collins, Daniel Dowd, Scot E. Colichio, Robert McDonnell, Kevin T. Green, Timothy TI Microbial Community in the Soil Determines the Forest Recovery Post-Exposure to Gamma Irradiation SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID BACTERIAL DIVERSITY; RADIATION; IMPACT; FUNGI AB Exposure of an ecosystem to ionizing radiation remains a possibility either due to accidents involving nuclear fuel rods or contamination with high-level radioactive wastes. While the short and long-term effect of ionizing radiation on higher eukaryotes has been well documented, we do not have an understanding on the recovery of the microbial community post radiation. Here we report that at a site within Brookhaven National Laboratory that was radiated from 1961 to 1978 with gamma rays (Gamma Forest), the ecosystem has not yet fully recovered from the effects of radiation. The current vegetation type in the Gamma Forest varies as one goes away from the source of ionizing radiation, with the region closest to the source having no vegetation. The microbial tag-encoded FLX amplicon pyrosequencing analysis of the soil from different regions suggests that the current microbial community structure is identical in all the Zones. When soil samples from each vegetation zone of the Gamma Forest were radiated with 1.8 kGy gamma radiation and survival microbial community analyzed, clear difference in the microbial communities were observed. It is evident based on the experimental data that the colonization of soil with Nitrosomonadaceae is critical for the higher plants in pine barrens to reestablish and grow after the area had been exposed to ionizing radiation. C1 [Shah, Vishal; Shah, Shreya; Collins, Daniel] Dowling Coll, Dept Biol, Oakdale, NY 11769 USA. [Mackey, Herman; Kambhampati, Murty] Southern Univ New Orleans, Dept Nat Sci, New Orleans, LA 70126 USA. [Colichio, Robert; Green, Timothy] Brookhaven Natl Lab, Upton, NY 11973 USA. [Dowd, Scot E.] Mol Res LP, Shallowater, TX 79363 USA. [McDonnell, Kevin T.] Dowling Coll, Dept Math & Comp Sci, Oakdale, NY 11769 USA. RP Shah, V (reprint author), Dowling Coll, Dept Biol, 150 Idle Hour Blvd, Oakdale, NY 11769 USA. EM shahv@dowling.edu FU NSF [CBET-1028438, HRD 0928797, DUE-0806894]; Foundation for Ecological Research in the Northeast; Dowling College FX This work was funded by grants from NSF (Grant # CBET-1028438) and The Foundation for Ecological Research in the Northeast to VS. HM and MK were supported through the NSF grants (HRD #0928797 and DUE-0806894). KM received support from the internal grants of Dowling College. NR 28 TC 0 Z9 0 U1 2 U2 29 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD OCT 15 PY 2013 VL 47 IS 20 BP 11396 EP 11402 DI 10.1021/es400923k PG 7 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA 240UQ UT WOS:000326123600006 PM 24063597 ER PT J AU Torkzaban, S Bradford, SA Wan, JM Tokunaga, T Masoudih, A AF Torkzaban, Saeed Bradford, Scott A. Wan, Jiamin Tokunaga, Tetsu Masoudih, Arash TI Release of Quantum Dot Nanoparticles in Porous Media: Role of Cation Exchange and Aging Time SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID COLLOID-FACILITATED TRANSPORT; TRANSIENT-CHEMICAL CONDITIONS; IONIC-STRENGTH; FULLERENE NANOPARTICLES; SOLUTION CHEMISTRY; GENETIC ALGORITHM; QUARTZ SANDS; DEPOSITION; MODEL; KINETICS AB Understanding the fate and transport of engineered nanoparticles (ENPs) in subsurface environments is required for developing the best strategy for waste management and disposal of these materials. In this study, the deposition and release of quantum dot (QD) nanoparticles were studied in saturated sand columns. The QDs were first deposited in columns using 100 mM NaCl or 2 mM CaCl2 solutions. Deposited QDs were then contacted with deionized (DI) water and/or varying Na+ concentrations to induce release. QDs deposited in 100 mM Na+ were easily reversible when the column was rinsed with DI water. Conversely, QDs deposited in the presence of Ca2+ exhibited resistance to release with DI water. However, significant release occurred when the columns were flushed with NaCl solutions. This release behavior was explained by cation exchange (Ca2+ in exchange sites were replaced by Na+) which resulted in the breakdown of calcium bridging. We also studied the effect of aging time on the QD release. As the aging time increased, smaller amounts of QDs were released following cation exchange. However, deposited QDs were subsequently released when the column was flushed with DI water. The release behavior was modeled using a single first-order kinetic release process and changes in the maximum solid phase concentration of deposited QDs with transition in solution chemistry. The results of this study demonstrate that the presence of carboxyl groups on ENPs and divalent ions in the solution plays a key role in controlling ENP mobility in the subsurface environment. C1 [Torkzaban, Saeed] CSIRO, Land & Water, Glen Osmond, SA 5064, Australia. [Bradford, Scott A.] ARS, USDA, US Salin Lab, Riverside, CA 92507 USA. [Wan, Jiamin; Tokunaga, Tetsu] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Masoudih, Arash] Catholic Univ Amer, Washington, DC 20064 USA. RP Torkzaban, S (reprint author), CSIRO, Land & Water, Glen Osmond, SA 5064, Australia. EM saeed.torkzaban@csiro.au RI Torkzaban, Saeed/G-7377-2013; Wan, Jiamin/H-6656-2014; Tokunaga, Tetsu/H-2790-2014; OI Torkzaban, Saeed/0000-0002-5146-9461; Tokunaga, Tetsu/0000-0003-0861-6128; Massoudieh, Arash/0000-0003-0200-2141 FU joint BER-EPA-NSF Nanoparticulate Research Program of the Office of Biological and Environmental Research, U.S. Department of Energy [DE-AC02-05CH11231] FX Funding was provided through the joint BER-EPA-NSF Nanoparticulate Research Program of the Office of Biological and Environmental Research, U.S. Department of Energy, under contract DE-AC02-05CH11231. NR 53 TC 22 Z9 22 U1 3 U2 52 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD OCT 15 PY 2013 VL 47 IS 20 BP 11528 EP 11536 DI 10.1021/es402075f PG 9 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA 240UQ UT WOS:000326123600022 PM 24041419 ER PT J AU Singer, DM Fox, PM Guo, H Marcus, MA Davis, JA AF Singer, David M. Fox, Patricia M. Guo, Hua Marcus, Matthew A. Davis, James A. TI Sorption and Redox Reactions of As(III) and As(V) within Secondary Mineral Coatings on Aquifer Sediment Grains SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID X-RAY-ABSORPTION; TRACER TEST; GRAVEL AQUIFER; CAPE-COD; GOETHITE; ADSORPTION; SAND; OXIDATION; ARSENIC(III); TRANSPORT AB Important reactive phenomena that affect the transport and fate of many elements occur at the mineral water interface (MINI), including sorption and redox reactions. Fundamental knowledge of these phenomena are often based on observations of ideal mineral water systems, for example, studies of molecular scale reactions on single crystal faces or the surfaces of pure mineral powders. Much less is understood about MINI in natural environments, which typically have nanometer to micrometer scale secondary mineral coatings on the surfaces of primary mineral grains. We examined sediment grain coatings from a well-characterized field site to determine the causes of rate limitations for arsenic (As) sorption and redox processes within the coatings. Sediments were obtained from the USGS field research site on Cape Cod, MA, and exposed to synthetic contaminated groundwater solutions. Uptake of As(III) and As(V) into the coatings was studied with a combination of electron microscopy and synchrotron techniques to assess concentration gradients and reactive processes, including electron transfer reactions. Transmission electron microscopy (TEM) and X-ray microprobe (XMP) analyses indicated that As was primarily associated with micrometer- to submicrometer aggregates of Mn-bearing nanoparticulate goethite. As(III) oxidation by this phase was observed but limited by the extent of exposed surface area of the goethite grains to the exterior of the mineral coatings. Secondary mineral coatings are potentially both sinks and sources of contaminants depending on the history of a contaminated site, and may need to be included explicitly in reactive transport models. C1 [Singer, David M.; Fox, Patricia M.; Davis, James A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Guo, Hua] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Marcus, Matthew A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Singer, DM (reprint author), Kent State Univ, Dept Geol, Kent, OH USA. EM dsinger4@kent.edu RI Foundry, Molecular/G-9968-2014; Fox, Patricia/I-2208-2014; Davis, James/G-2788-2015 OI Fox, Patricia/0000-0002-5264-1876; FU Laboratory Directed Research and Development (LDRD) and Sustainable Systems (SS) Scientific Focus Area (SPA); Office of Science, of the U.S. Department of Energy [DE-AC02-05CH11231]; U.S. DOE [DE-AC02-06CH11357]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; U.S. Department of Energy [DE-AC02-05CH11231] FX We gratefully acknowledge support from the Laboratory Directed Research and Development (LDRD) and Sustainable Systems (SS) Scientific Focus Area (SPA) funding at Lawrence Berkeley National Laboratory, provided by the Director, Office of Science, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Portions of this work were carried out at the Stanford Synchrotron Radiation Lightsource (SSRL) and the National Center for Electron Microscopy (NCEM) at Lawrence Berkeley National Laboratory (LBNL). We thank Joern Larsen (LBL) for ICP analyses, Nazi la Kaviani (USGS) for BET analyses, and Sam Webb (SSRL), Benjamin Kocar (SSRL), Matthew Newville (APS), Joanne Stubbs (APS), and Ruth Tinnacher (LBL) for XMP data collection assistance. SSRL is a Directorate of SLAC National Accelerator Laboratory and an Office of Science User Facility operated for the U.S. Department of Energy Office of Science by Stanford University. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NCEM is supported by the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Comments from three anonymous reviewers improved this manuscript. NR 52 TC 9 Z9 9 U1 5 U2 58 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD OCT 15 PY 2013 VL 47 IS 20 BP 11569 EP 11576 DI 10.1021/es402754f PG 8 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA 240UQ UT WOS:000326123600027 PM 24041305 ER PT J AU Gilmour, CC Podar, M Bullock, AL Graham, AM Brown, SD Somenahally, AC Johs, A Hurt, RA Bailey, KL Elias, DA AF Gilmour, Cynthia C. Podar, Mircea Bullock, Allyson L. Graham, Andrew M. Brown, Steven D. Somenahally, Anil C. Johs, Alex Hurt, Richard A., Jr. Bailey, Kathryn L. Elias, Dwayne A. TI Mercury Methylation by Novel Microorganisms from New Environments SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID SULFATE-REDUCING BACTERIA; PSYCHROPHILUS SP-NOV.; GEN. NOV.; METHYLMERCURY PRODUCTION; GEOBACTER-SULFURREDUCENS; AQUATIC ECOSYSTEMS; WASTE-WATER; METHANOGEN; RICE; BIOAVAILABILITY AB Microbial mercury (Hg) methylation transforms a toxic trace metal into the highly bioaccumulated neurotoxin methylmercury (MeHg). The lack of a genetic marker for microbial MeHg production has prevented a dear understanding of Hg-methylating organism distribution in nature. Recently, a specific gene cluster (hgcAB) was linked to Hg methylation in two bacteria.(1) Here we test if the presence of hgcAB orthologues is a reliable predictor of Hg methylation capability in microorganisms, a necessary confirmation for the development of molecular probes for Hg-methylation in nature. Although hgcAB orthologues are rare among all available microbial genomes, organisms are much more phylogenetically and environmentally diverse than previously thought. By directly measuring MeHg production in several bacterial and archaeal strains encoding hgcAB, we confirmed that possessing hgcAB predicts Hg methylation capability. For the first time, we demonstrated Hg methylation in a number of species other than sulfate- (SRB) and iron- (FeRB) reducing bacteria, including methanogens, and syntrophic, acetogenic, and fermentative Firmicutes. Several of these species occupy novel environmental niches for Hg methylation, including methanogenic habitats such as rice paddies, the animal gut, and extremes of pH and salinity. Identification of these organisms as Hg methylators now links methylation to discrete gene markers in microbial communities. C1 [Gilmour, Cynthia C.; Bullock, Allyson L.] Smithsonian Environm Res Ctr, Edgewater, MD 21037 USA. [Podar, Mircea; Brown, Steven D.; Somenahally, Anil C.; Hurt, Richard A., Jr.; Bailey, Kathryn L.; Elias, Dwayne A.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. [Johs, Alex] Oak Ridge Natl Lab, Environm Sci Div, Oak Ridge, TN 37831 USA. [Graham, Andrew M.] Grinnell Coll, Grinnell, IA 50112 USA. RP Elias, DA (reprint author), Oak Ridge Natl Lab, Biosci Div, POB 2008,MS 6036, Oak Ridge, TN 37831 USA. EM eliasda@ornl.gov RI Elias, Dwayne/B-5190-2011; Johs, Alexander/F-1229-2011; Brown, Steven/A-6792-2011; Gilmour, Cynthia/G-1784-2010; OI Elias, Dwayne/0000-0002-4469-6391; Johs, Alexander/0000-0003-0098-2254; Brown, Steven/0000-0002-9281-3898; Gilmour, Cynthia/0000-0002-1720-9498; Podar, Mircea/0000-0003-2776-0205 FU Subsurface Biogeochemical Research Program (SBR) within the U.S. Department of Energy, Office of Science, Biological and Environmental Research; Smithsonian Environmental Research Center; SBR; National Science Foundation [DEB0351050]; U.S. Department of Energy [DEAC05-00OR22725] FX This research was conducted by the Oak Ridge National Laboratory Mercury Subsurface Science Focus Area with support from the Subsurface Biogeochemical Research Program (SBR) within the U.S. Department of Energy, Office of Science, Biological and Environmental Research and by the Smithsonian Environmental Research Center with support from SBR and National Science Foundation Grant DEB0351050 to C.G. ORNL is managed by UT-Battelle LLC for the U.S. Department of Energy under contract DEAC05-00OR22725. We thank Robert Sanford for A. dehalogens strain K, Mike McInerney for S. acidotrophicus, and Joel Kostka for G. daltonii. Andrew Maizel, Taylan Morcol, Alyssa Wetterauer, and Georgia Riedel performed all mercury analyses at SERC. NR 67 TC 103 Z9 105 U1 24 U2 182 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD OCT 15 PY 2013 VL 47 IS 20 BP 11810 EP 11820 DI 10.1021/es403075t PG 11 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA 240UQ UT WOS:000326123600056 PM 24024607 ER PT J AU Clark, CE Horner, RM Harto, CB AF Clark, Corrie E. Horner, Robert M. Harto, Christopher B. TI Life Cycle Water Consumption for Shale Gas and Conventional Natural Gas SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID MANAGEMENT AB Shale gas production represents a large potential source of natural gas for the nation. The scale and rapid growth in shale gas development underscore the need to better understand its environmental implications, including water consumption. This study estimates the water consumed over the life cycle of conventional and shale gas production, accounting for the different stages of production and for flowback water reuse (in the case of shale gas). This study finds that shale gas consumes more water over its life cycle (13-37 L/GJ) than conventional natural gas consumes (9.3-9.6 L/GJ). However, when used as a transportation fuel, shale gas consumes significantly less water than other transportation fuels. When used for electricity generation, the combustion of shale gas adds incrementally to the overall water consumption compared to conventional natural gas. The impact of fuel production, however, is small relative to that of power plant operations. The type of power plant where the natural gas is utilized is far more important than the source of the natural gas. C1 [Clark, Corrie E.; Horner, Robert M.; Harto, Christopher B.] Argonne Natl Lab, Div Environm Sci, Washington, DC 20024 USA. RP Clark, CE (reprint author), Argonne Natl Lab, Div Environm Sci, 955 LEnfant Plaza SW,Suite 6000, Washington, DC 20024 USA. EM ceclark@anl.gov RI Harto, Christopher/D-9573-2013 FU U.S. Department of Energy [DE-AC02-06CH11357] FX This study was supported by the U.S. Department of Energy under Contract No. DE-AC02-06CH11357. NR 40 TC 39 Z9 41 U1 9 U2 82 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD OCT 15 PY 2013 VL 47 IS 20 BP 11829 EP 11836 DI 10.1021/es4013855 PG 8 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA 240UQ UT WOS:000326123600058 PM 24004382 ER PT J AU Kraiem, M Essex, RM Mathew, KJ Orlowicz, GJ Soriano, MD AF Kraiem, M. Essex, R. M. Mathew, K. J. Orlowicz, G. J. Soriano, M. D. TI Re-certification of the CRM 125-A UO2 fuel pellet standard for uranium isotopic composition SO INTERNATIONAL JOURNAL OF MASS SPECTROMETRY LA English DT Article DE Uranium; Certified reference material; TIMS; Isotope-amount ratio; Total evaporation; Conventional analyses AB The U.S. Department of Energy New Brunswick Laboratory (NBL) has been tasked to develop certified reference materials (CRMs) tailored for the demands of modern analytical methods in the field of nuclear forensics. As part of this effort, several existing uranium CRMs are being characterized for additional attributes. One of these materials is the CRM 125-A uranium oxide (UO2) pellet assay and isotopic standard (4% enriched in U-235), which is being developed as a CRM for U-Th age determinations. Reliable U isotopic composition data with relatively small uncertainties are essential for use as a uranium age standard. Therefore, re-characterization of the uranium isotopic composition of CRM 125-A was deemed necessary due to poorly constrained minor U abundances (i.e., U-234 and U-236) resulting from instrumental limitations of the mass spectrometer used at the time of original certification (1996-1997). The analytical work presented in this study was undertaken with the purpose of reducing the uncertainties of certificate values for uranium isotope-amount ratios. Six randomly selected CRM 125-A pellets were characterized for the uranium isotopic abundances by thermal ionization mass spectrometry (TIMS). The re-certified major ratio n(U-235)/n(U-238) of 0.042301(25) was determined using the total evaporation (TE) and modified total evaporation (MTE) methods. The re-certified minor isotope ratios n( U-234)/n(U-238) and n(U-238)/n(U-238) of 0.00039130(38) and 0.0000040754(47), respectively, were measured by MTE and a conventional Faraday cup analysis method using internal normalization. Additionally, the material was checked for the presence of U-233 using a secondary electron multiplier (SEM) equipped with a retarding potential quadrupole (RPQ). No U-233 was observed within the instrumental detection limit. The homogeneity of CRM 125-A was confirmed by the absence of any statistically significant unit-to-unit variation in the uranium isotope amount ratios. The new values measured in this study represent a considerable refinement of the older data, in particular for the minor ratios, with uncertainties that are significantly smaller than those cited in the original certificate. The results of the characterization analyses are presented along with an explanation of the uncertainty estimates, which are compliant with the Guide to the Expression of Uncertainty in Measurement (GUM). (C) 2013 Elsevier B.V. All rights reserved. C1 [Kraiem, M.; Essex, R. M.; Mathew, K. J.; Orlowicz, G. J.; Soriano, M. D.] US DOE, New Brunswick Lab, Argonne, IL 60439 USA. RP Kraiem, M (reprint author), IAEA, Vienna Int Ctr, POB 100, A-1400 Vienna, Austria. EM M.Kraiem@iaea.org FU National Technical Nuclear Forensics Center (NTNFC) of the Department of Homeland Security (DHS) under Inter-Agency Agreement [HSHQDC-10-X-00135]; U.S. Department of Energy (DOE) FX This work was supported by the National Technical Nuclear Forensics Center (NTNFC) of the Department of Homeland Security (DHS) under Inter-Agency Agreement HSHQDC-10-X-00135, and by an appointment to the New Brunswick Laboratory (NBL) Research Participation Program sponsored by the U.S. Department of Energy (DOE) and administered by the Oak Ridge Institute for Science and Education (ORISE). The authors wish to thank their colleagues U.I. Narayanan and C. Gradle for comments on the draft paper that helped improve the overall quality of the manuscript. NR 13 TC 4 Z9 4 U1 2 U2 13 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 1387-3806 EI 1873-2798 J9 INT J MASS SPECTROM JI Int. J. Mass Spectrom. PD OCT 15 PY 2013 VL 352 BP 37 EP 43 DI 10.1016/j.ijms.2013.05.007 PG 7 WC Physics, Atomic, Molecular & Chemical; Spectroscopy SC Physics; Spectroscopy GA 236WP UT WOS:000325830500005 ER PT J AU Camarillo, MK Stringfellow, WT Spier, CL Hanlon, JS Domen, JK AF Camarillo, Mary Kay Stringfellow, William T. Spier, Chelsea L. Hanlon, Jeremy S. Domen, Jeremy K. TI Impact of co-digestion on existing salt and nutrient mass balances for a full-scale dairy energy project SO JOURNAL OF ENVIRONMENTAL MANAGEMENT LA English DT Article DE Dairy manure; Anaerobic digestion; Co-digestion; Salinity; Nutrients ID ANAEROBIC-DIGESTION; BIOGAS PRODUCTION; TRACE COMPOUNDS; PLANTS; WASTE; MANURE; CROPS; FARM; AVAILABILITY; OPERATIONS AB Anaerobic digestion of manure and other agricultural waste streams with subsequent energy production can result in more sustainable dairy operations; however, importation of digester feedstocks onto dairy farms alters previously established carbon, nutrient, and salinity mass balances. Salt and nutrient mass balance must be maintained to avoid groundwater contamination and salination. To better understand salt and nutrient contributions of imported methane-producing substrates, a mass balance for a full-scale dairy biomass energy project was developed for solids, carbon, nitrogen, sulfur, phosphorus, chloride, and potassium. Digester feedstocks, consisting of thickened manure flush-water slurry, screened manure solids, sudan grass silage, and feed-waste, were tracked separately in the mass balance. The error in mass balance closure for most elements was less than 5%. Manure contributed 69.2% of influent dry matter while contributing 77.7% of nitrogen, 90.9% of sulfur, and 73.4% of phosphorus. Sudan grass silage contributed high quantities of chloride and potassium, 33.3% and 43.4%, respectively, relative to the dry matter contribution of 22.3%. Five potential off-site co-digestates (egg waste, grape pomace, milk waste, pasta waste, whey wastewater) were evaluated for anaerobic digestion based on salt and nutrient content in addition to bio-methane potential. Egg waste and wine grape pomace appeared the most promising co-digestates due to their high methane potentials relative to bulk volume. Increasing power production from the current rate of 369 kW to the design value of 710 kW would require co-digestion with either 26800 L d(-1) egg waste or 60900 kg d(-1) grape pomace. However, importation of egg waste would more than double nitrogen loading, resulting in an increase of 172% above the baseline while co-digestion with grape pomace would increase potassium by 279%. Careful selection of imported co-digestates and management of digester effluent is required to manage salt and nutrient mass loadings and reduce groundwater impacts. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Camarillo, Mary Kay; Stringfellow, William T.] Univ Pacific, Dept Civil Engn, Sch Engn & Comp Sci, Stockton, CA 95211 USA. [Camarillo, Mary Kay; Stringfellow, William T.; Spier, Chelsea L.; Hanlon, Jeremy S.; Domen, Jeremy K.] Univ Pacific, Ecol Engn Res Program, Sch Engn & Comp Sci, Stockton, CA 95211 USA. [Stringfellow, William T.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Camarillo, MK (reprint author), Univ Pacific, Dept Civil Engn, Sch Engn & Comp Sci, 3601 Pacific Ave, Stockton, CA 95211 USA. EM mcamarillo@pacific.edu RI Stringfellow, William/O-4389-2015 OI Stringfellow, William/0000-0003-3189-5604 FU US Department of Energy National Energy Technology Laboratory [DE-EE0001895]; California Energy Commission [PIR-10-053] FX Funding was received from the US Department of Energy National Energy Technology Laboratory, Assistance Agreement DE-EE0001895 and from the California Energy Commission, Contract Number #PIR-10-053. Laboratory and field assistance was received from Matthew Ebia, Michael Jue, Cameron Ross, and Ashley Stubblefield. NR 41 TC 3 Z9 3 U1 4 U2 59 PU ACADEMIC PRESS LTD- ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL RD, LONDON NW1 7DX, ENGLAND SN 0301-4797 EI 1095-8630 J9 J ENVIRON MANAGE JI J. Environ. Manage. PD OCT 15 PY 2013 VL 128 BP 233 EP 242 DI 10.1016/j.jenvman.2013.04.060 PG 10 WC Environmental Sciences SC Environmental Sciences & Ecology GA 241YA UT WOS:000326203400027 PM 23747374 ER PT J AU Lanekoff, I Burnum-Johnson, K Thomas, M Short, J Carson, JP Cha, J Dey, SK Yang, PX Conaway, MCP Laskin, J AF Lanekoff, Ingela Burnum-Johnson, Kristin Thomas, Mathew Short, Joshua Carson, James P. Cha, Jeeyeon Dey, Sudhansu K. Yang, Pengxiang Conaway, Maria C. Prieto Laskin, Julia TI High-Speed Tandem Mass Spectrometric in Situ Imaging by Nanospray Desorption Electrospray Ionization Mass Spectrometry SO ANALYTICAL CHEMISTRY LA English DT Article ID COMPLEX ORGANIC MIXTURES; THIN TISSUE-SECTIONS; STRUCTURAL-CHARACTERIZATION; ATMOSPHERIC-PRESSURE; DRUG DISTRIBUTION; MOUSE-BRAIN; ION-SOURCE; RAT-BRAIN; METABOLITES; GLYCEROPHOSPHOLIPIDS AB Nanospray desorption electrospray ionization (nano-DESI) combined with tandem mass spectrometry (MS/MS), high-resolution mass analysis of the fragment ions (m/Delta m = 17 500 at m/z 200), and rapid spectral acquisition enabled simultaneous imaging and identification of a large number of metabolites and lipids from 92 selected m/z windows (+/- 1 Da) with a spatial resolution of better than 150 pm. Mouse uterine sections of implantation sites on day 6 of pregnancy were analyzed in the ambient environment without any sample pretreatment. MS/MS imaging was performed by scanning the sample under the nano-DESI probe at 10 mu m/s, while higher-energy collision-induced dissociation (HCD) spectra were acquired for a targeted inclusion list of 92 m/z values at a rate of similar to 6.3 spectra/s. Molecular ions and their corresponding fragments, separated by high-resolution mass analysis, were assigned on the basis of accurate mass measurement. Using this approach, we were able to identify and image both abundant and low-abundance isobaric and isomeric species within each m/z window. MS/MS analysis enabled efficient separation and identification of isomeric and isobaric phospholipids that are difficult to separate in full-scan mode. Furthermore, we identified several metabolites associated with early pregnancy and obtained the first 2D images of these molecules. C1 [Lanekoff, Ingela; Short, Joshua; Laskin, Julia] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. [Burnum-Johnson, Kristin; Thomas, Mathew; Carson, James P.] Pacific NW Natl Lab, Biol Sci Div, Richland, WA 99352 USA. [Cha, Jeeyeon; Dey, Sudhansu K.] Univ Cincinnati, Div Reprod Sci, Perinatal Inst, Cincinnati Childrens Hosp Med Ctr,Coll Med, Cincinnati, OH 45229 USA. [Yang, Pengxiang; Conaway, Maria C. Prieto] Thermo Fisher Sci, San Jose, CA 95134 USA. RP Lanekoff, I (reprint author), Pacific NW Natl Lab, Div Phys Sci, POB 999,K8-88, Richland, WA 99352 USA. EM Julia.Laskin@pnnl.gov RI Burnum, Kristin/B-1308-2011; Laskin, Julia/H-9974-2012 OI Burnum, Kristin/0000-0002-2722-4149; Laskin, Julia/0000-0002-4533-9644 FU U.S. Department of Energy (DOE) [DE-AC05-76RL01830]; DOE's Office of Biological and Environmental Research; NIH [HD068524, DA06668]; Ruth L. Kirschstein predoctoral NRSA fellowship [F30AG040858] FX The research described in this paper is part of the Chemical Imaging Initiative at Pacific Northwest National Laboratory (PNNL). It was conducted under the Laboratory Directed Research and Development Program at PNNL a multiprogram national laboratory operated by Battelle for the U.S. Department of Energy (DOE) under Contract DE-AC05-76RL01830. The research was performed at EMSL, a national scientific user facility sponsored by the DOE's Office of Biological and Environmental Research and located at PNNL. This work was partially supported by NIH grants (HD068524 and DA06668 to S.K.D.), and J.C. is supported by a Ruth L. Kirschstein predoctoral NRSA fellowship (F30AG040858). NR 71 TC 22 Z9 23 U1 11 U2 102 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0003-2700 EI 1520-6882 J9 ANAL CHEM JI Anal. Chem. PD OCT 15 PY 2013 VL 85 IS 20 BP 9596 EP 9603 DI 10.1021/ac401760s PG 8 WC Chemistry, Analytical SC Chemistry GA 240VU UT WOS:000326126600026 PM 24040919 ER PT J AU Ge, XX Tao, Y Zhang, AD Lin, YH Du, D AF Ge, Xiaoxiao Tao, Yuan Zhang, Aidong Lin, Yuehe Du, Dan TI Electrochemical Detection of Dual Exposure Biomarkers of Organophosphorus Agents Based on Reactivation of Inhibited Cholinesterase SO ANALYTICAL CHEMISTRY LA English DT Article ID NERVE AGENTS; MASS-SPECTROMETRY; PHOSPHORYLATED ACETYLCHOLINESTERASE; ENZYME-ACTIVITY; PESTICIDES; ASSAY; BUTYRYLCHOLINESTERASE; QUANTIFICATION; IMMUNOSENSOR; THIOCHOLINE AB Considering inter- or intra-individual variation in the normal levels of acetylcholinesterase (AChE), real-time measurement of AChE via the reactivation from a postexposure sample was used, and thus a baseline-free and reliable approach was proposed for detecting/screening low-dose organophosphorus pesticides (OPs) poisons. The principle of this technology is on the basis of parallel measurements of AChE activity before and after reactivation from a postexposure to simultaneously provide the content of dual biomarkers of both enzyme inhibition and enzyme adducts. It is more accurate and reliable compared with only one biomarker (inhibition or adduct). Reactivation from a postexposure sample is a better individual enzyme baseline compared to pre-exposure from the population average level in currently available approaches. AChE activity was measured with an electrochemical method. Greatly enhanced sensitivity was achieved by using Fe3O4/Au nanocomposites to enrich thiocholine, the hydrolysis product of active AChE, followed by electrochemical oxidative desorption of the adsorbed thiocholine. The validation of this method for measurement of OP exposures was further explored with in vitro paraoxon inhibited human red blood cells (RBCs) samples and demonstrated its practicability. C1 [Ge, Xiaoxiao; Tao, Yuan; Zhang, Aidong; Du, Dan] Cent China Normal Univ, Key Lab Pesticide & Chem Biol, Minist Educ, Coll Chem, Wuhan 430079, Hubei, Peoples R China. [Lin, Yuehe; Du, Dan] Washington State Univ, Sch Mech & Mat Engn, Pullman, WA 99164 USA. [Lin, Yuehe] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Du, D (reprint author), Cent China Normal Univ, Key Lab Pesticide & Chem Biol, Minist Educ, Coll Chem, Wuhan 430079, Hubei, Peoples R China. EM dan.du@mail.ccnu.edu.cn RI Du, Dan (Annie)/G-3821-2012; Lin, Yuehe/D-9762-2011 OI Lin, Yuehe/0000-0003-3791-7587 FU National Natural Science Foundation of China [21275062, 21075047]; Program for New Century Excellent Talents in University [NCET-12-0871]; U.S. DOE [DE-AC05-76RL01830] FX This work was supported by the National Natural Science Foundation of China (21275062, 21075047) and the Program for New Century Excellent Talents in University (NCET-12-0871). Pacific Northwest National Laboratory is operated by Battelle for U.S. DOE under contract DE-AC05-76RL01830. NR 36 TC 20 Z9 20 U1 7 U2 67 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0003-2700 EI 1520-6882 J9 ANAL CHEM JI Anal. Chem. PD OCT 15 PY 2013 VL 85 IS 20 BP 9686 EP 9691 DI 10.1021/ac402022p PG 6 WC Chemistry, Analytical SC Chemistry GA 240VU UT WOS:000326126600038 PM 24020883 ER PT J AU Baran, R Northen, TR AF Baran, Richard Northen, Trent R. TI Robust Automated Mass Spectra Interpretation and Chemical Formula Calculation Using Mixed Integer Linear Programming SO ANALYTICAL CHEMISTRY LA English DT Article ID SYNECHOCOCCUS-SP. PCC-7002; METABOLITE IDENTIFICATION; DATA SETS; SPECTROMETRY; METABOLOMICS; OPTIMIZATION; ANNOTATION; REVEALS; RULES AB Untargeted metabolite profiling using liquid chromatography and mass spectrometry coupled via electrospray ionization is a powerful tool for the discovery of novel natural products, metabolic capabilities, and biomarkers. However, the elucidation of the identities of uncharacterized metabolites from spectral features remains challenging. A critical step in the metabolite identification workflow is the assignment of redundant spectral features (adducts, fragments, multimers) and calculation of the underlying chemical formula. Inspection of the data by experts using computational tools solving partial problems (e.g., chemical formula calculation for individual ions) can be performed to disambiguate alternative solutions and provide reliable results. However, manual curation is tedious and not readily scalable or standardized. Here we describe an automated procedure for the robust automated mass spectra interpretation and chemical formula calculation using mixed integer linear programming optimization (RAMSI). Chemical rules among related ions are expressed as linear constraints and both the spectra interpretation and chemical formula calculation are performed in a single optimization step. This approach is unbiased in that it does not require predefined sets of neutral losses and positive and negative polarity spectra can be combined in a single optimization. The procedure was evaluated with 30 experimental mass spectra and was found to effectively identify the protonated or deprotonated molecule ([M + H](+) or [M - H](-)) while being robust to the presence of background ions. RAMSI provides a much-needed standardized tool for interpreting ions for subsequent identification in untargeted metabolomics workflows. C1 [Baran, Richard; Northen, Trent R.] Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. RP Northen, TR (reprint author), Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. EM TRNorthen@lbl.gov OI Northen, Trent/0000-0001-8404-3259 FU Office of Science, Office of Biological and Environmental Research, of the U.S. Department of Energy [DE-AC02-05CH11231] FX We thank Kai Duhrkop for performing chemical formula calculations with our test data using SIRIUS. This work was conducted by ENIGMA-Ecosystems and Networks Integrated with Genes and Molecular Assemblies Program from the Office of Biological and Environmental Research of the U.S. Department of Energy supported by the Office of Science, Office of Biological and Environmental Research, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 27 TC 2 Z9 2 U1 1 U2 29 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0003-2700 EI 1520-6882 J9 ANAL CHEM JI Anal. Chem. PD OCT 15 PY 2013 VL 85 IS 20 BP 9777 EP 9784 DI 10.1021/ac402180c PG 8 WC Chemistry, Analytical SC Chemistry GA 240VU UT WOS:000326126600051 PM 24032353 ER PT J AU Schroll, CA Chatterjee, S Levitskaia, TG Heineman, WR Bryan, SA AF Schroll, Cynthia A. Chatterjee, Sayandev Levitskaia, Tatiana G. Heineman, William R. Bryan, Samuel A. TI Electrochemistry and Spectroelectrochemistry of Europium(III) Chloride in 3LiCl-2KCl from 643 to 1123 K SO ANALYTICAL CHEMISTRY LA English DT Article ID KCL EUTECTIC SALT; LICL-KCL; THERMODYNAMIC PROPERTIES; CYCLIC VOLTAMMETRY; MOLTEN NACL-2CSCL; REDOX EQUILIBRIUM; IONS; ACTINIDES; BEHAVIOR; URANIUM AB The electrochemical and spectroelectrochemical behavior of europium(III) chloride in a molten salt eutectic, 3LiCl-2KCl, over a temperature range of 643-1123 K using differential pulse voltammetry, cyclic voltammetry, potential step chronoabsorptometry, and thin-layer spectroelectrochemistry is reported. The electrochemical reaction was determined to be the one-electron reduction of Eu3+ to Eu2+ at all temperatures. The redox potential of Eu3+/2+ shifts to more positive potentials, and the diffusion coefficient for Eu3+ increases as temperature increases. The results for the number of electrons transferred, redox potential, and diffusion coefficient are in good agreement between the electrochemical and spectroelectrochemical techniques. This research extends our ability to develop a spectroelectrochemical sensor for lanthanides and actinides into molten salt media. C1 [Schroll, Cynthia A.; Heineman, William R.] Univ Cincinnati, Dept Chem, Cincinnati, OH 45221 USA. [Chatterjee, Sayandev; Levitskaia, Tatiana G.; Bryan, Samuel A.] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. RP Heineman, WR (reprint author), Univ Cincinnati, Dept Chem, Cincinnati, OH 45221 USA. EM william.heineman@uc.edu; sam.bryan@pnnl.gov RI Bryan, Samuel/D-5457-2015; OI Bryan, Samuel/0000-0001-5664-3249; Chatterjee, Sayandev/0000-0003-2218-5635 FU U.S. Department of Energy's Fuel Cycle Research and Development (FCR&D), Separation Campaign (NE); U.S. Department of Energy [DE-AC05-76RL01830] FX This research was supported by the U.S. Department of Energy's Fuel Cycle Research and Development (FCR&D), Separation Campaign (NE) and performed at the Pacific Northwest National Laboratory operated by Battelle for the U.S. Department of Energy under Contract DE-AC05-76RL01830. NR 57 TC 7 Z9 7 U1 2 U2 33 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0003-2700 EI 1520-6882 J9 ANAL CHEM JI Anal. Chem. PD OCT 15 PY 2013 VL 85 IS 20 BP 9924 EP 9931 DI 10.1021/ac402518p PG 8 WC Chemistry, Analytical SC Chemistry GA 240VU UT WOS:000326126600070 PM 24016214 ER PT J AU Denton, JS Murrell, MT Goldstein, SJ Nunn, AJ Amato, RS Hinrichs, KA AF Denton, J. S. Murrell, M. T. Goldstein, S. J. Nunn, A. J. Amato, R. S. Hinrichs, K. A. TI Evaluation of New Geological Reference Materials for Uranium-Series Measurements: Chinese Geological Standard Glasses (CGSG) and Macusanite Obsidian SO ANALYTICAL CHEMISTRY LA English DT Article ID MASS-SPECTROMETRY; U-SERIES; ISOTOPE RATIOS; MAGMA GENESIS; MC-ICPMS; TH; FEMTOSECOND; U-238; GEOCHEMISTRY; TRANSPORT AB Recent advances in high-resolution, rapid, in situ microanalytical techniques present numerous opportunities for the analytical community, provided accurately characterized reference materials are available. Here, we present multicollector thermal ionization mass spectrometry (MC-TIMS) and multicollector inductively coupled plasma mass spectrometry (MC-ICP-MS) uranium and thorium concentration and isotopic data obtained by isotope dilution for a suite of newly available Chinese Geological Standard Glasses (CGSG) designed for microanalysis. These glasses exhibit a range of compositions including basalt, syenite, andesite, and a soil. Uranium concentrations for these glasses range. from similar to 2 to 14 mu g g(-1), Th/U weight ratios range from similar to 4 to 6, U-234/U-238 activity ratios range from 0.93 to 1.02, and Th-230/U-238 activity ratios range from 0.98 to 1.12. Uranium and thorium concentration and isotopic data are also presented for a rhyolitic obsidian from Macusani, SE Peru (macusanite). This glass can also be used as a rhyolitic reference material, has a very low Th/U weight ratio (around 0.077), and is approximately in U-238-U-234-Th-230 secular equilibrium. The U-Th concentration data agree with but are significantly more precise than those previously measured. U-Th concentration and isotopic data agree within estimated errors for the two measurement techniques, providing validation of the two methods. The large U-238-U-234-Th-230 disequilibria for some of the glasses, along with the wide range in their chemical compositions and Th/U ratios should provide useful reference points for the U-series analytical community. C1 [Denton, J. S.; Murrell, M. T.; Goldstein, S. J.; Nunn, A. J.; Amato, R. S.; Hinrichs, K. A.] Los Alamos Natl Lab, Nucl & Radiochem C NR, Los Alamos, NM 87545 USA. RP Denton, JS (reprint author), Sellafield Ltd, Sellafield, Seascale CA20 1PG, Cumbria, England. EM joanna.s.denton@sellafieldsites.com OI Hinrichs, Kimberly/0000-0002-4881-5204 FU Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences and Biosciences Division of the U.S. Department of Energy [2013LANLE3CC] FX The authors would like to thank Xiuchun Zhan (National Research Centre for Geoanalysis, China) and Anastassia Borisova (Geosciences Observatory, University of Toulouse, France for providing the reference materials. We also thank two anonymous reviewers whose comments provided clarity to the manuscript. This research was supported by Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences and Biosciences Division of the U.S. Department of Energy under Contract No. 2013LANLE3CC to Los Alamos National Laboratory. NR 50 TC 4 Z9 5 U1 0 U2 20 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0003-2700 EI 1520-6882 J9 ANAL CHEM JI Anal. Chem. PD OCT 15 PY 2013 VL 85 IS 20 BP 9975 EP 9981 DI 10.1021/ac4017117 PG 7 WC Chemistry, Analytical SC Chemistry GA 240VU UT WOS:000326126600077 PM 24004454 ER PT J AU Lees, JP Poireau, V Tisserand, V Grauges, E Palano, A Eigen, G Stugu, B Brown, DN Kerth, LT Kolomensky, YG Lee, MJ Lynch, G Koch, H Schroeder, T Hearty, C Mattison, TS McKenna, JA So, RY Khan, A Blinov, VE Buzykaev, AR Druzhinin, VP Golubev, VB Kravchenko, EA Onuchin, AP Serednyakov, SI Skovpen, YI Solodov, EP Todyshev, KY Yushkov, AN Kirkby, D Lankford, AJ Mandelkern, M Dey, B Gary, JW Long, O Vitug, GM Campagnari, C Sevilla, MF Hong, TM Kovalskyi, D Richman, JD West, CA Eisner, AM Lockman, WS Martinez, AJ Schumm, BA Seiden, A Chao, DS Cheng, CH Echenard, B Flood, KT Hitlin, DG Ongmongkolkul, P Porter, FC Andreassen, R Huard, Z Meadows, BT Pushpawela, BG Sokoloff, MD Sun, L Bloom, PC Ford, WT Gaz, A Nagel, M Nauenberg, U Smith, JG Wagner, SR Ayad, R Toki, WH Spaan, B Schwierz, R Bernard, D Verderi, M Playfer, S Bettoni, D Bozzi, C Calabrese, R Cibinetto, G Fioravanti, E Garzia, I Luppi, E Piemontese, L Santoro, V Baldini-Ferroli, R Calcaterra, A de Sangro, R Finocchiaro, G Martellotti, S Patteri, P Peruzzi, IM Piccolo, M Rama, M Zallo, A Contri, R Guido, E Lo Vetere, M Monge, MR Passaggio, S Patrignani, C Robutti, E Bhuyan, B Prasad, V Morii, M Adametz, A Uwer, U Lacker, HM Dauncey, PD Mallik, U Chen, C Cochran, J Meyer, WT Prell, S Rubin, AE Gritsan, AV Arnaud, N Davier, M Derkach, D Grosdidier, G Le Diberder, F Lutz, AM Malaescu, B Roudeau, P Stocchi, A Wormser, G Lange, DJ Wright, DM Coleman, JP Fry, JR Gabathuler, E Hutchcroft, DE Payne, DJ Touramanis, C Bevan, AJ Di Lodovico, F Sacco, R Cowan, G Bougher, J Brown, DN Davis, CL Denig, AG Fritsch, M Gradl, W Griessinger, K Hafner, A Prencipe, E Schubert, KR Barlow, RJ Lafferty, GD Behn, E Cenci, R Hamilton, B Jawahery, A Roberts, DA Cowan, R Dujmic, D Sciolla, G Cheaib, R Patel, PM Robertson, SH Biassoni, P Neri, N Palombo, F Cremaldi, L Godang, R Sonnek, P Summers, DJ Nguyen, X Simard, M Taras, P De Nardo, G Monorchio, D Onorato, G Sciacca, C Martinelli, M Raven, G Jessop, CP LoSecco, JM Honscheid, K Kass, R Brau, J Frey, R Sinev, NB Strom, D Torrence, E Feltresi, E Margoni, M Morandin, M Posocco, M Rotondo, M Simi, G Simonetto, F Stroili, R Akar, S Ben-Haim, E Bomben, M Bonneaud, GR Briand, H Calderini, G Chauveau, J Leruste, P Marchiori, G Ocariz, J Sitt, S Biasini, M Manoni, E Pacetti, S Rossi, A Angelini, C Batignani, G Bettarini, S Carpinelli, M Casarosa, G Cervelli, A Forti, F Giorgi, MA Lusiani, A Oberhof, B Paoloni, E Perez, A Rizzo, G Walsh, JJ Pegna, DL Olsen, J Smith, AJS Faccini, R Ferrarotto, F Ferroni, F Gaspero, M Gioi, LL Piredda, G Bunger, C Grunberg, O Hartmann, T Leddig, T Voss, C Waldi, R Adye, T Olaiya, EO Wilson, FF Emery, S de Monchenault, GH Vasseur, G Yeche, C Anulli, F Aston, D Bard, DJ Benitez, JF Cartaro, C Convery, MR Dorfan, J Dubois-Felsmann, GP Dunwoodie, W Ebert, M Field, RC Fulsom, BG Gabareen, AM Graham, MT Hast, C Innes, WR Kim, P Kocian, ML Leith, DWGS Lewis, P Lindemann, D Lindquist, B Luitz, S Luth, V Lynch, HL MacFarlane, DB Muller, DR Neal, H Nelson, S Perl, M Pulliam, T Ratcliff, BN Roodman, A Salnikov, AA Schindler, RH Snyder, A Su, D Sullivan, MK Va'vra, J Wagner, AP Wang, WF Wisniewski, WJ Wittgen, M Wright, DH Wulsin, HW Ziegler, V Park, W Purohit, MV White, RM Wilson, JR Randle-Conde, A Sekula, SJ Bellis, M Burchat, PR Miyashita, TS Puccio, EMT Alam, MS Ernst, JA Gorodeisky, R Guttman, N Peimer, DR Soffer, A Spanier, SM Ritchie, JL Ruland, AM Schwitters, RF Wray, BC Izen, JM Lou, XC Bianchi, F De Mori, F Filippi, A Gamba, D Zambito, S Lanceri, L Vitale, L Martinez-Vidal, F Oyanguren, A Villanueva-Perez, P Ahmed, H Albert, J Banerjee, S Bernlochner, FU Choi, HHF King, GJ Kowalewski, R Lewczuk, MJ Lueck, T Nugent, IM Roney, JM Sobie, RJ Tasneem, N Gershon, TJ Harrison, PF Latham, TE Band, HR Dasu, S Pan, Y Prepost, R Wu, SL AF Lees, J. P. Poireau, V. Tisserand, V. Grauges, E. Palano, A. Eigen, G. Stugu, B. Brown, D. N. Kerth, L. T. Kolomensky, Yu. G. Lee, M. J. Lynch, G. Koch, H. Schroeder, T. Hearty, C. Mattison, T. S. McKenna, J. A. So, R. Y. Khan, A. Blinov, V. E. Buzykaev, A. R. Druzhinin, V. P. Golubev, V. B. Kravchenko, E. A. Onuchin, A. P. Serednyakov, S. I. Skovpen, Yu. I. Solodov, E. P. Todyshev, K. Yu. Yushkov, A. N. Kirkby, D. Lankford, A. J. Mandelkern, M. Dey, B. Gary, J. W. Long, O. Vitug, G. M. Campagnari, C. Sevilla, M. Franco Hong, T. M. Kovalskyi, D. Richman, J. D. West, C. A. Eisner, A. M. Lockman, W. S. Martinez, A. J. Schumm, B. A. Seiden, A. Chao, D. S. Cheng, C. H. Echenard, B. Flood, K. T. Hitlin, D. G. Ongmongkolkul, P. Porter, F. C. Andreassen, R. Huard, Z. Meadows, B. T. Pushpawela, B. G. Sokoloff, M. D. Sun, L. Bloom, P. C. Ford, W. T. Gaz, A. Nagel, M. Nauenberg, U. Smith, J. G. Wagner, S. R. Ayad, R. Toki, W. H. Spaan, B. Schwierz, R. Bernard, D. Verderi, M. Playfer, S. Bettoni, D. Bozzi, C. Calabrese, R. Cibinetto, G. Fioravanti, E. Garzia, I. Luppi, E. Piemontese, L. Santoro, V. Baldini-Ferroli, R. Calcaterra, A. de Sangro, R. Finocchiaro, G. Martellotti, S. Patteri, P. Peruzzi, I. M. Piccolo, M. Rama, M. Zallo, A. Contri, R. Guido, E. Lo Vetere, M. Monge, M. R. Passaggio, S. Patrignani, C. Robutti, E. Bhuyan, B. Prasad, V. Morii, M. Adametz, A. Uwer, U. Lacker, H. M. Dauncey, P. D. Mallik, U. Chen, C. Cochran, J. Meyer, W. T. Prell, S. Rubin, A. E. Gritsan, A. V. Arnaud, N. Davier, M. Derkach, D. Grosdidier, G. Le Diberder, F. Lutz, A. M. Malaescu, B. Roudeau, P. Stocchi, A. Wormser, G. Lange, D. J. Wright, D. M. Coleman, J. P. Fry, J. R. Gabathuler, E. Hutchcroft, D. E. Payne, D. J. Touramanis, C. Bevan, A. J. Di Lodovico, F. Sacco, R. Cowan, G. Bougher, J. Brown, D. N. Davis, C. L. Denig, A. G. Fritsch, M. Gradl, W. Griessinger, K. Hafner, A. Prencipe, E. Schubert, K. R. Barlow, R. J. Lafferty, G. D. Behn, E. Cenci, R. Hamilton, B. Jawahery, A. Roberts, D. A. Cowan, R. Dujmic, D. Sciolla, G. Cheaib, R. Patel, P. M. Robertson, S. H. Biassoni, P. Neri, N. Palombo, F. Cremaldi, L. Godang, R. Sonnek, P. Summers, D. J. Nguyen, X. Simard, M. Taras, P. De Nardo, G. Monorchio, D. Onorato, G. Sciacca, C. Martinelli, M. Raven, G. Jessop, C. P. LoSecco, J. M. Honscheid, K. Kass, R. Brau, J. Frey, R. Sinev, N. B. Strom, D. Torrence, E. Feltresi, E. Margoni, M. Morandin, M. Posocco, M. Rotondo, M. Simi, G. Simonetto, F. Stroili, R. Akar, S. Ben-Haim, E. Bomben, M. Bonneaud, G. R. Briand, H. Calderini, G. Chauveau, J. Leruste, Ph. Marchiori, G. Ocariz, J. Sitt, S. Biasini, M. Manoni, E. Pacetti, S. Rossi, A. Angelini, C. Batignani, G. Bettarini, S. Carpinelli, M. Casarosa, G. Cervelli, A. Forti, F. Giorgi, M. A. Lusiani, A. Oberhof, B. Paoloni, E. Perez, A. Rizzo, G. Walsh, J. J. Pegna, D. Lopes Olsen, J. Smith, A. J. S. Faccini, R. Ferrarotto, F. Ferroni, F. Gaspero, M. Gioi, L. Li Piredda, G. Buenger, C. Gruenberg, O. Hartmann, T. Leddig, T. Voss, C. Waldi, R. Adye, T. Olaiya, E. O. Wilson, F. F. Emery, S. de Monchenault, G. Hamel Vasseur, G. Yeche, Ch. Anulli, F. Aston, D. Bard, D. J. Benitez, J. F. Cartaro, C. Convery, M. R. Dorfan, J. Dubois-Felsmann, G. P. Dunwoodie, W. Ebert, M. Field, R. C. Fulsom, B. G. Gabareen, A. M. Graham, M. T. Hast, C. Innes, W. R. Kim, P. Kocian, M. L. Leith, D. W. G. S. Lewis, P. Lindemann, D. Lindquist, B. Luitz, S. Luth, V. Lynch, H. L. MacFarlane, D. B. Muller, D. R. Neal, H. Nelson, S. Perl, M. Pulliam, T. Ratcliff, B. N. Roodman, A. Salnikov, A. A. Schindler, R. H. Snyder, A. Su, D. Sullivan, M. K. Va'vra, J. Wagner, A. P. Wang, W. F. Wisniewski, W. J. Wittgen, M. Wright, D. H. Wulsin, H. W. Ziegler, V. Park, W. Purohit, M. V. White, R. M. Wilson, J. R. Randle-Conde, A. Sekula, S. J. Bellis, M. Burchat, P. R. Miyashita, T. S. Puccio, E. M. T. Alam, M. S. Ernst, J. A. Gorodeisky, R. Guttman, N. Peimer, D. R. Soffer, A. Spanier, S. M. Ritchie, J. L. Ruland, A. M. Schwitters, R. F. Wray, B. C. Izen, J. M. Lou, X. C. Bianchi, F. De Mori, F. Filippi, A. Gamba, D. Zambito, S. Lanceri, L. Vitale, L. Martinez-Vidal, F. Oyanguren, A. Villanueva-Perez, P. Ahmed, H. Albert, J. Banerjee, Sw. Bernlochner, F. U. Choi, H. H. F. King, G. J. Kowalewski, R. Lewczuk, M. J. Lueck, T. Nugent, I. M. Roney, J. M. Sobie, R. J. Tasneem, N. Gershon, T. J. Harrison, P. F. Latham, T. E. Band, H. R. Dasu, S. Pan, Y. Prepost, R. Wu, S. L. CA BABAR Collaboration TI Measurement of the B+ -> omega l(+) nu branching fraction with semileptonically tagged B mesons SO PHYSICAL REVIEW D LA English DT Article ID BABAR DETECTOR; DECAYS AB We report a measurement of the branching fraction of the exclusive charmless semileptonic decay B+ -> omega l(+) nu, where l is either an electron or amuon. We use samples of B+ mesons tagged by a reconstructed charmed semileptonic decay of the other B meson in the event. The measurement is based on a data set of 426.1 fb(-1) of e(+)e(-) collisions at a center-of-mass energy of 10.58 GeV recorded with the BABAR detector at the PEP-II asymmetric-energy e(+)e(-) storage rings. We measure a branching fraction of B(B+ -> omega l(+) nu) = (1.35 +/- 0.21 +/- 0.11) x 10(-4), where the uncertainties are statistical and systematic, respectively. We also present measurements of the partial branching fractions in three bins of q(2), the invariant-mass squared of the lepton-neutrino system, and we compare them to theoretical predictions of the form factors. C1 [Lees, J. P.; Poireau, V.; Tisserand, V.] Univ Savoie, Lab Annecy Le Vieux Phys Particules LAPP, CNRS, IN2P3, F-74941 Annecy Le Vieux, France. [Grauges, E.] Univ Barcelona, Fac Fis, Dept ECM, E-08028 Barcelona, Spain. [Palano, A.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Palano, A.] Univ Bari, Dipartimento Fis, I-70126 Bari, Italy. 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[Buenger, C.; Gruenberg, O.; Hartmann, T.; Leddig, T.; Voss, C.; Waldi, R.] Univ Rostock, D-18051 Rostock, Germany. [Adye, T.; Olaiya, E. O.; Wilson, F. F.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Emery, S.; de Monchenault, G. Hamel; Vasseur, G.; Yeche, Ch.] CEA, Irfu, SPP, Ctr Saclay, F-91191 Gif Sur Yvette, France. [Anulli, F.; Aston, D.; Bard, D. J.; Benitez, J. F.; Cartaro, C.; Convery, M. R.; Dorfan, J.; Dubois-Felsmann, G. P.; Dunwoodie, W.; Ebert, M.; Field, R. C.; Fulsom, B. G.; Gabareen, A. M.; Graham, M. T.; Hast, C.; Innes, W. R.; Kim, P.; Kocian, M. L.; Leith, D. W. G. S.; Lewis, P.; Lindemann, D.; Lindquist, B.; Luitz, S.; Luth, V.; Lynch, H. L.; MacFarlane, D. B.; Muller, D. R.; Neal, H.; Nelson, S.; Perl, M.; Pulliam, T.; Ratcliff, B. N.; Roodman, A.; Salnikov, A. A.; Schindler, R. H.; Snyder, A.; Su, D.; Sullivan, M. K.; Va'vra, J.; Wagner, A. P.; Wang, W. F.; Wisniewski, W. J.; Wittgen, M.; Wright, D. H.; Wulsin, H. W.; Ziegler, V.] SLAC Natl Accelerator Lab, Stanford, CA 94309 USA. [Park, W.; Purohit, M. V.; White, R. M.; Wilson, J. R.] Univ S Carolina, Columbia, SC 29208 USA. [Randle-Conde, A.; Sekula, S. J.] So Methodist Univ, Dallas, TX 75275 USA. [Bellis, M.; Burchat, P. R.; Miyashita, T. S.; Puccio, E. M. T.] Stanford Univ, Stanford, CA 94305 USA. [Alam, M. S.; Ernst, J. A.] SUNY Albany, Albany, NY 12222 USA. [Gorodeisky, R.; Guttman, N.; Peimer, D. R.; Soffer, A.] Tel Aviv Univ, Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Spanier, S. M.] Univ Tennessee, Knoxville, TN 37996 USA. [Ritchie, J. L.; Ruland, A. M.; Schwitters, R. F.; Wray, B. C.] Univ Texas Austin, Austin, TX 78712 USA. [Izen, J. M.; Lou, X. C.] Univ Texas Dallas, Richardson, TX 75083 USA. [Bianchi, F.; De Mori, F.; Filippi, A.; Gamba, D.; Zambito, S.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Bianchi, F.; De Mori, F.; Gamba, D.; Zambito, S.] Univ Turin, Dipartimento Fis Sperimentale, I-10125 Turin, Italy. [Lanceri, L.; Vitale, L.] Ist Nazl Fis Nucl, Sez Trieste, I-34127 Trieste, Italy. [Lanceri, L.; Vitale, L.] Univ Trieste, Dipartimento Fis, I-34127 Trieste, Italy. [Martinez-Vidal, F.; Oyanguren, A.; Villanueva-Perez, P.] Univ Valencia, CSIC, IFIC, E-46071 Valencia, Spain. [Ahmed, H.; Albert, J.; Banerjee, Sw.; Bernlochner, F. U.; Choi, H. H. F.; King, G. J.; Kowalewski, R.; Lewczuk, M. J.; Lueck, T.; Nugent, I. M.; Roney, J. M.; Sobie, R. J.; Tasneem, N.] Univ Victoria, Victoria, BC V8W 3P6, Canada. [Gershon, T. J.; Harrison, P. F.; Latham, T. E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Band, H. R.; Dasu, S.; Pan, Y.; Prepost, R.; Wu, S. L.] Univ Wisconsin, Madison, WI 53706 USA. [Carpinelli, M.] Univ Sassari, I-07100 Sassari, Italy. RP Nagel, M (reprint author), Univ Colorado, Boulder, CO 80309 USA. EM nagel@mpp.mpg.de RI Lusiani, Alberto/A-3329-2016; Morandin, Mauro/A-3308-2016; Di Lodovico, Francesca/L-9109-2016; Calcaterra, Alessandro/P-5260-2015; Frey, Raymond/E-2830-2016; White, Ryan/E-2979-2015; Kravchenko, Evgeniy/F-5457-2015; Calabrese, Roberto/G-4405-2015; Martinez Vidal, F*/L-7563-2014; Kolomensky, Yury/I-3510-2015; Lo Vetere, Maurizio/J-5049-2012; Lusiani, Alberto/N-2976-2015; Patrignani, Claudia/C-5223-2009; Monge, Maria Roberta/G-9127-2012; Forti, Francesco/H-3035-2011; Oyanguren, Arantza/K-6454-2014; Luppi, Eleonora/A-4902-2015 OI Lusiani, Alberto/0000-0002-6876-3288; Morandin, Mauro/0000-0003-4708-4240; Di Lodovico, Francesca/0000-0003-3952-2175; Calcaterra, Alessandro/0000-0003-2670-4826; Frey, Raymond/0000-0003-0341-2636; White, Ryan/0000-0003-3589-5900; Calabrese, Roberto/0000-0002-1354-5400; Martinez Vidal, F*/0000-0001-6841-6035; Kolomensky, Yury/0000-0001-8496-9975; Lo Vetere, Maurizio/0000-0002-6520-4480; Lusiani, Alberto/0000-0002-6876-3288; Patrignani, Claudia/0000-0002-5882-1747; Monge, Maria Roberta/0000-0003-1633-3195; Forti, Francesco/0000-0001-6535-7965; Oyanguren, Arantza/0000-0002-8240-7300; Luppi, Eleonora/0000-0002-1072-5633 FU DOE (U.S.); NSF (U.S.); NSERC (Canada); CEA (France); CNRS-IN2P3 (France); BMBF (Germany); DFG (Germany); INFN (Italy); FOM (The Netherlands); NFR (Norway); MES (Russia); MINECO (Spain); STFC (U.K.); Marie Curie EIF (European Union); A.P. Sloan Foundation (U.S.) FX We are grateful for the excellent luminosity and machine conditions provided by our PEP-II colleagues, and for the substantial dedicated effort from the computing organizations that support BABAR. The collaborating institutions wish to thank SLAC for its support and kind hospitality. This work is supported by DOE and NSF (U.S.), NSERC (Canada), CEA and CNRS-IN2P3 (France), BMBF and DFG (Germany), INFN (Italy), FOM (The Netherlands), NFR (Norway), MES (Russia), MINECO (Spain), STFC (U.K.). Individuals have received support from the Marie Curie EIF (European Union) and the A.P. Sloan Foundation (U.S.). NR 22 TC 7 Z9 7 U1 0 U2 15 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD OCT 15 PY 2013 VL 88 IS 7 AR 072006 DI 10.1103/PhysRevD.88.072006 PG 8 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 240MD UT WOS:000326099800002 ER PT J AU Bouchard, C Lepage, GP Monahan, C Na, HC Shigemitsu, J AF Bouchard, Chris Lepage, G. Peter Monahan, Christopher Na, Heechang Shigemitsu, Junko CA HPQCD Collaboration TI Standard Model Predictions for B -> Kl(+)l(-) with Form Factors from Lattice QCD SO PHYSICAL REVIEW LETTERS LA English DT Article ID HEAVY AB We calculate, for the first time using unquenched lattice QCD form factors, the standard model differential branching fractions dB/dq(2) (B -> Kl(+)l(-)) for l = e, mu, tau and compare with experimental measurements by Belle, BABAR, CDF, and LHCb. We report on B(B -> Kl(+)l(-)) in q(2) bins used by experiment and predict B(B -> K tau(+)tau(-)) = (1.41 +/- 0.15) x 10(-7). We also calculate the ratio of branching fractions R-e(mu) = 1.00029(69) and predict R-l(tau) = 1.176(40), for l = e, mu. Finally, we calculate the "flat term" in the angular distribution of the differential decay rate F-H(e,mu,tau) in experimentally motivated q(2) bins. C1 [Bouchard, Chris; Shigemitsu, Junko] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. [Lepage, G. Peter] Cornell Univ, Lab Elementary Particle Phys, Ithaca, NY 14853 USA. [Monahan, Christopher] Coll William & Mary, Dept Phys, Williamsburg, VA 23187 USA. [Na, Heechang] Argonne Natl Lab, Argonne Leadership Comp Facil, Argonne, IL 60439 USA. RP Bouchard, C (reprint author), Ohio State Univ, Dept Phys, 174 W 18th Ave, Columbus, OH 43210 USA. EM bouchard.18@osu.edu RI Bouchard, Christopher/N-3723-2016 OI Bouchard, Christopher/0000-0003-1639-7164 FU DOE; NSF; Office of Science of the U.S. DOE FX This research was supported by the DOE and NSF. We thank the MILC collaboration for making their asqtad Nf = 2 + 1 gauge field configurations available. Computations were carried out at the Ohio Supercomputer Center and on facilities of the USQCD collaboration funded by the Office of Science of the U.S. DOE. NR 40 TC 39 Z9 39 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 15 PY 2013 VL 111 IS 16 AR 162002 DI 10.1103/PhysRevLett.111.162002 PG 5 WC Physics, Multidisciplinary SC Physics GA 240TI UT WOS:000326119500002 PM 24182256 ER PT J AU Nguyen, MC Choi, JH Zhao, X Wang, CZ Zhang, Z Ho, KM AF Nguyen, Manh Cuong Choi, Jin-Ho Zhao, Xin Wang, Cai-Zhuang Zhang, Zhenyu Ho, Kai-Ming TI New Layered Structures of Cuprous Chalcogenides as Thin Film Solar Cell Materials: Cu2Te and Cu2Se SO PHYSICAL REVIEW LETTERS LA English DT Article ID AUGMENTED-WAVE METHOD; AB-INITIO DATA; EFFECTIVE POTENTIALS; OPTIMIZATION; EFFICIENCY; METALS AB The stable crystal structures of two cuprous chalcogenides of Cu2X (X = Te or Se) are predicted using an adaptive genetic algorithm in combination with first-principles density functional theory calculations. Both systems are found to prefer a unique and previously unrecognized layered structure, with the total energies much lower than all structures proposed in the literature so far. The newly discovered structures are further shown to be dynamically and mechanically stable, and possess electronic properties consistent with existing experimental observations. In particular, their layered nature is expected to prevail over other structural forms at the interfaces of thin-film solar cells, and knowledge about the precise atomic structures of the interfaces is a prerequisite for achieving long-term stability and high efficiency of CdTe and Cu(In, Ga)Se-2 solar cells. C1 [Nguyen, Manh Cuong; Zhao, Xin; Wang, Cai-Zhuang; Ho, Kai-Ming] Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. [Nguyen, Manh Cuong; Zhao, Xin; Wang, Cai-Zhuang; Ho, Kai-Ming] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Choi, Jin-Ho; Zhang, Zhenyu; Ho, Kai-Ming] Univ Sci & Technol China, Int Ctr Quantum Design Funct Mat ICQD, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Peoples R China. RP Nguyen, MC (reprint author), Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. EM zhangzy@ustc.edu.cn; kmh@ameslab.gov RI Nguyen, Manh Cuong/G-2783-2015; OI Nguyen, Manh Cuong/0000-0001-8027-9029; Zhao, Xin/0000-0002-3580-512X FU U.S. Department of Energy, Office of Basic Energy Science, Division of Materials Science and Engineering [DE-AC02-07CH11358]; NRF [2012R1A6A3A03040199]; NSFC [11034006, 11250110056] FX The U.S. Department of Energy, Office of Basic Energy Science, Division of Materials Science and Engineering supported the research, including GA development, at the Ames Laboratory, which is operated for the DOE by Iowa State University under Contract No. DE-AC02-07CH11358, with an additional computing grant through the National Energy Research Scientific Computing Center (NERSC). The work was also partially supported from Korea (J.-H. C., NRF Grant No. 2012R1A6A3A03040199) and China (J.-H. C. and Z. Z., NSFC Grants No. 11034006 and No. 11250110056). M. C. N. and J.-H. C. contributed equally to this work. NR 38 TC 24 Z9 25 U1 12 U2 113 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 15 PY 2013 VL 111 IS 16 AR 165502 DI 10.1103/PhysRevLett.111.165502 PG 5 WC Physics, Multidisciplinary SC Physics GA 240TI UT WOS:000326119500007 PM 24182279 ER PT J AU Li, T Zan, XJ Sun, Y Zuo, XB Li, XD Senesi, A Winans, RE Wang, Q Lee, B AF Li, Tao Zan, Xingjie Sun, Yong Zuo, Xiaobing Li, Xiaodong Senesi, Andrew Winans, Randall E. Wang, Qian Lee, Byeongdu TI Self-Assembly of Rodlike Virus to Superlattices SO LANGMUIR LA English DT Article ID TOBACCO-MOSAIC-VIRUS; NANOPARTICLE SUPERLATTICES; NANOCRYSTAL SUPERLATTICES; M13 BACTERIOPHAGE; ELECTRIC-FIELD; ALKALINE PH; PARTICLES; METHYLCELLULOSE; WATER; CRYSTALLIZATION AB Rodlike tobacco mosaic virus (TMV) has been found to assemble into superlattices in aqueous solution using the polymer methylcellulose to induce depletion and free volume entropy-based attractive forces. Both transmission electron microscopy and small-angle X-ray scattering show that the superlattices form in both semidilute and concentrated regimes of polymer, where the free volume entropy and the depletion interaction are the dominant driving force, respectively. The superlattices are NaCl and temperature responsive. The rigidity of the rodlike nanoparticles also plays an important role for the formation of superlattices through the free volume entropy mechanism. Compared to the rigid TMV particle, flexible bacteriophage M13 particles are only responsive to the depletion force and thus only assemble in highly concentrated polymer solution, where depletion interaction is dominant. C1 [Li, Tao; Zuo, Xiaobing; Senesi, Andrew; Winans, Randall E.; Lee, Byeongdu] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. [Zan, Xingjie; Wang, Qian] Univ S Carolina, Dept Chem & Biochem, Columbia, SC 29208 USA. [Sun, Yong; Li, Xiaodong] Univ S Carolina, Dept Mech Engn, Columbia, SC 29208 USA. RP Wang, Q (reprint author), Univ S Carolina, Dept Chem & Biochem, 631 Sumter St, Columbia, SC 29208 USA. EM wang263@mailbox.sc.edu; blee@aps.anl.gov RI li, tao/K-8911-2012; OI li, tao/0000-0001-5454-1468; Wang, Qian/0000-0002-2149-384X; Lee, Byeongdu/0000-0003-2514-8805 FU U.S. DOE [DE-AC02-06CH11357]; US NSF [CHE-0748690, DMR-0706431, CMMI-1129979, CMMI-0968843] FX We are thankful for the use of Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract DE-AC02-06CH11357. Q Wang is grateful for the financial support from the US NSF CHE-0748690 and US NSF DMR-0706431. Y. Sun and X. D. Li thank the financial support from the U.S. National Science Foundation (CMMI-1129979 and CMMI-0968843). NR 57 TC 5 Z9 5 U1 5 U2 74 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0743-7463 EI 1520-5827 J9 LANGMUIR JI Langmuir PD OCT 15 PY 2013 VL 29 IS 41 BP 12777 EP 12784 DI 10.1021/la402933q PG 8 WC Chemistry, Multidisciplinary; Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA 240UP UT WOS:000326123500021 PM 24044529 ER PT J AU Abelev, B Adam, J Adamova, D Adare, AM Aggarwal, MM Rinella, GA Agnello, M Agocs, AG Agostinelli, A Ahammed, Z Ahmad, N Masoodi, AA Ahn, SA Ahn, SU Ajaz, M Akindinov, A Aleksandrov, D Alessandro, B Alici, A Alkin, A Avina, EA Alme, J Alt, T Altini, V Altinpinar, S Altsybeev, I Andrei, C Andronic, A Anguelov, V Anielski, J Anson, C Anticic, T Antinori, F Antonioli, P Aphecetche, L Appelshauser, H Arbor, N Arcelli, S Arend, A Armesto, N Arnaldi, R Aronsson, T Arsene, IC Arslandok, M Asryan, A Augustinus, A Averbeck, R Awes, TC Aysto, J Azmi, MD Bach, M Badala, A Baek, YW Bailhache, R Bala, R Baldisseri, A Pedrosa, FBD Ban, J Baral, RC Barbera, R Barile, F Barnafoldi, GG Barnby, LS Barret, V Bartke, J Basile, M Bastid, N Basu, S Bathen, B Batigne, G Batyunya, B Baumann, C Bearden, IG Beck, H Behera, NK Belikov, I Bellini, F Bellwied, R Belmont-Moreno, E Bencedi, G Beole, S Berceanu, I Bercuci, A Berdnikov, Y Berenyi, D Bergognon, AAE Berzano, D Betev, L Bhasin, A Bhati, AK Bhom, J Bianchi, L Bianchi, N Bielcik, J Bielcikova, J Bilandzic, A Bjelogrlic, S Blanco, F Blanco, F Blau, D Blume, C Boccioli, M Bottger, S Bogdanov, A Boggild, H Bogolyubsky, M Boldizsar, L Bombara, M Book, J Borel, H Borissov, A Bossu, F Botje, M Botta, E Braidot, E Braun-Munzinger, P Bregant, M Breitner, T Broker, TA Browning, TA Broz, M Brun, R Bruna, E Bruno, GE Budnikov, D Buesching, H Bufalino, S Buncic, P Busch, O Buthelezi, Z Caffarri, D Cai, X Caines, H Villar, EC Camerini, P Roman, VC Romeo, GC Carena, F Carena, W Carlin, N Carminati, F Diaz, AC Castellanos, JC Hernandez, JFC Casula, EAR Catanescu, V Cavicchioli, C Sanchez, CC Cepila, J Cerello, P Chang, B Chapeland, S Charvet, JL Chattopadhyay, S Chattopadhyay, S Cherney, M Cheshkov, C Cheynis, B Barroso, VC Chinellato, DD Chochula, P Chojnacki, M Choudhury, S Christakoglou, P Christensen, CH Christiansen, P Chujo, T Chung, SU Cicalo, C Cifarelli, L Cindolo, F Cleymans, J Colamaria, F Colella, D Collu, A Balbastre, GC del Valle, ZC Connors, ME Contin, G Contreras, JG Cormier, M Morales, YC Cortese, P Maldonado, IC Cosentino, MR Costa, F Cotallo, ME Crescio, E Crochet, P Alaniz, EC Albino, RC Cuautle, E Cunqueiro, L Dainese, A Danu, A Das, K Das, I Das, S Das, D Dash, S Dash, A De, S de Barros, GOV De Caro, A de Cataldo, G de Cuveland, J De Falco, A De Gruttola, D Delagrange, H Delagrange, H De Marco, N Denes, E De Pasquale, S Deppman, A Erasmo, GD de Rooij, R Corchero, MAD Di Bari, D Dietel, T Di Giglio, C Di Liberto, S Di Mauro, A Di Nezza, P Divia, R Djuvsland, O Dobrin, A Dobrowolski, T Donigus, B Dordic, O Driga, O Dubey, AK Dubla, A Ducroux, L Dupieux, P Majumdar, AKD Elia, D Emschermann, D Engel, H Erazmus, B Erdal, HA Espagnon, B Estienne, M Esumi, S Evans, D Eyyubova, G Fabris, D Faivre, J Falchieri, D Fantoni, A Fasel, M Fearick, R Fehlker, D Feldkamp, L Felea, D Feliciello, A Fenton-Olsen, B Feofilov, G Tellez, AF Ferretti, A Festanti, A Figiel, J Figueredo, MAS Filchagin, S Finogeev, D Fionda, FM Fiore, EM Floratos, E Floris, M Foertsch, S Foka, P Fokin, S Fragiacomo, E Francescon, A Frankenfeld, U Fuchs, U Furget, C Girard, MF Gaardhoje, JJ Gagliardi, M Gago, A Gallio, M Gangadharan, DR Ganoti, P Garabatos, C Garcia-Solis, E Gargiulo, C Garishvili, I Gerhard, J Germain, M Geuna, C Gheata, A Gheata, M Ghidini, B Ghosh, P Gianotti, P Girard, MR Giubellino, P Gladysz-Dziadus, E Glassel, P Gomez, R Ferreiro, EG Gonzalez-Trueba, LH Gonzalez-Zamora, P Gorbunov, S Goswami, A Gotovac, S Graczykowski, LK Grajcarek, R Grelli, A Grigoras, A Grigoras, C Grigoriev, V Grigoryan, S Grigoryan, A Grinyov, B Grion, N Gros, P Grosse-Oetringhaus, JF Grossiord, JY Grosso, R Guber, F Guernane, R Guerzoni, B Guilbaud, M Gulbrandsen, K Gulkanyan, H Gunji, T Gupta, R Gupta, A Haake, R Haaland, O Hadjidakis, C Haiduc, M Hamagaki, H Hamar, G Han, BH Hanratty, LD Hansen, A Harmanova-Tothova, Z Harris, JW Hartig, M Harton, A Hatzifotiadou, D Hayashi, S Hayrapetyan, A Heckel, ST Heide, M Helstrup, H Herghelegiu, A Corral, GH Herrmann, N Hess, BA Hetland, KF Hicks, B Hippolyte, B Hori, Y Hristov, P Hrivnacova, I Huang, M Humanic, TJ Hwang, DS Ichou, R Ilkaev, R Ilkiv, I Inaba, M Incani, E Innocenti, GM Innocenti, PG Ippolitov, M Irfan, M Ivan, C Ivanov, M Ivanov, A Ivanov, V Ivanytskyi, O Jacholkowski, A Jacobs, PM Jang, HJ Janik, MA Janik, R Jayarathna, PHSY Jena, S Jha, DM Bustamante, RTJ Jones, PG Jung, H Jusko, A Kaidalov, AB Kalcher, S Kalinak, P Kalliokoski, T Kalweit, A Kang, JH Kaplin, V Uysal, AK Karavichev, O Karavicheva, T Karpechev, E Kazantsev, A Kebschull, U Keidel, R Khan, MM 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CA ALICE Collaboration TI Centrality dependence of pi, K, and p production in Pb-Pb collisions at root s(NN)=2.76 TeV SO PHYSICAL REVIEW C LA English DT Article ID HEAVY-ION COLLISIONS; QUARK-GLUON PLASMA; NUCLEUS-NUCLEUS COLLISIONS; QCD PHASE-TRANSITION; TOTAL CROSS-SECTIONS; CHEMICAL FREEZE-OUT; HADRON-PRODUCTION; COLLABORATION; PERSPECTIVE; MODELS AB In this paper measurements are presented of pi(+/-), K-+/-, p, and (p) over bar production at midrapidity (vertical bar y vertical bar < 0.5), in Pb-Pb collisions at root s(NN) = 2.76 TeV as a function of centrality. The measurement covers the transverse-momentum (p(T)) range from 100, 200, and 300 MeV/c up to 3, 3, and 4.6 GeV/c for pi, K, and p, respectively. The measured p(T) distributions and yields are compared to expectations based on hydrodynamic, thermal and recombination models. The spectral shapes of central collisions show a stronger radial flow than measured at lower energies, which can be described in hydrodynamic models. 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[Gunji, T.; Hamagaki, H.; Hayashi, S.; Hori, Y.; Ozawa, K.; Torii, H.; Tsuji, T.; Yamaguchi, Y.] Univ Tokyo, Tokyo, Japan. [Han, B. H.; Hwang, D. S.; Kim, S.; Kim, J. H.; Son, H.] Sejong Univ, Dept Phys, Seoul, South Korea. [Hess, B. A.; Schmidt, H. R.; Wiechula, J.] Univ Tubingen, Tubingen, Germany. [Kalweit, A.; Mager, M.; Oeschler, H.] Tech Univ Darmstadt, Inst Kernphys, Darmstadt, Germany. [Uysal, A. Karasu] Yildiz Tech Univ, Istanbul, Turkey. [Uysal, A. Karasu] KTO Karatay Univ, Konya, Turkey. [Keidel, R.] Fachhochschule Worms, ZTT, Worms, Germany. [Klay, J. L.] Calif Polytech State Univ San Luis Obispo, San Luis Obispo, CA 93407 USA. [Knospe, A. G.; Markert, C.; Karampatsos, L. Xaplanteris] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Lemmon, R. C.; Romita, R.] STFC Daresbury Lab, Nucl Phys Grp, Daresbury, England. [Malinina, L.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Mares, J.; Polak, K.; Zavada, P.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Martashvili, I.; Mazer, J.; Nattrass, C.; Read, K. F.; Scott, R.; Sharma, N.] Univ Tennessee, Knoxville, TN USA. [Meddi, F.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Milosevic, J.] Univ Belgrade, Fac Phys, YU-11001 Belgrade, Serbia. [Milosevic, J.] Univ Belgrade, Vinca Inst Nucl Sci, YU-11001 Belgrade, Serbia. [Mishra, A. N.; Sahoo, R.] Indian Inst Technol Indore, Indore, Madhya Pradesh, India. [Mohanty, B.; Singha, S.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Pestov, Y.] Budker Inst Nucl Phys, Novosibirsk 630090, Russia. [Redlich, K.] Univ Wroclaw, Inst Theoret Phys, PL-50138 Wroclaw, Poland. [Ricci, R. A.; Vannucci, L.] Ist Nazl Fis Nucl, Lab Nazl Legnaro, I-35020 Legnaro, Italy. [Sakaguchi, H.; Shigaki, K.; Sugitate, T.] Hiroshima Univ, Hiroshima, Japan. [Ulrich, J.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Vernet, R.] Ctr Calcul IN2P3, Villeurbanne, France. RP Abelev, B (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RI Bielcikova, Jana/G-9342-2014; Adamova, Dagmar/G-9789-2014; Barnby, Lee/G-2135-2010; Blau, Dmitry/H-4523-2012; Yang, Hongyan/J-9826-2014; Cosentino, Mauro/L-2418-2014; Bearden, Ian/M-4504-2014; Sumbera, Michal/O-7497-2014; Felea, Daniel/C-1885-2012; Barnafoldi, Gergely Gabor/L-3486-2013; Peitzmann, Thomas/K-2206-2012; Kharlov, Yuri/D-2700-2015; Krizek, Filip/G-8967-2014; feofilov, grigory/A-2549-2013; Kovalenko, Vladimir/C-5709-2013; Castillo Castellanos, Javier/G-8915-2013; Levai, Peter/A-1544-2014; Takahashi, Jun/B-2946-2012; Guber, Fedor/I-4271-2013; Martinez Davalos, Arnulfo/F-3498-2013; Bregant, Marco/I-7663-2012; Wagner, Vladimir/G-5650-2014; Sevcenco, Adrian/C-1832-2012; Vajzer, Michal/G-8469-2014; Suaide, Alexandre/L-6239-2016; Deppman, Airton/J-5787-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Ferreiro, Elena/C-3797-2017; Armesto, Nestor/C-4341-2017; Ferretti, Alessandro/F-4856-2013; Martinez Hernandez, Mario Ivan/F-4083-2010; Vickovic, Linda/F-3517-2017; Fernandez Tellez, Arturo/E-9700-2017; Vechernin, Vladimir/J-5832-2013; Janik, Malgorzata/O-7520-2015; Graczykowski, Lukasz/O-7522-2015; Christensen, Christian/D-6461-2012; De Pasquale, Salvatore/B-9165-2008; Chinellato, David/D-3092-2012; de Cuveland, Jan/H-6454-2016; Kurepin, Alexey/H-4852-2013; Jena, Deepika/P-2873-2015; Akindinov, Alexander/J-2674-2016; Nattrass, Christine/J-6752-2016; Mitu, Ciprian/E-6733-2011; Usai, Gianluca/E-9604-2015; Salgado, Carlos A./G-2168-2015; Bruna, Elena/C-4939-2014; Karasu Uysal, Ayben/K-3981-2015; HAMAGAKI, HIDEKI/G-4899-2014; Pshenichnov, Igor/A-4063-2008; Kompaniets, Mikhail/F-5025-2013; Altsybeev, Igor/K-6687-2013; Vinogradov, Leonid/K-3047-2013; Kondratiev, Valery/J-8574-2013 OI Gago Medina, Alberto Martin/0000-0002-0019-9692; Dainese, Andrea/0000-0002-2166-1874; Paticchio, Vincenzo/0000-0002-2916-1671; Monteno, Marco/0000-0002-3521-6333; Bhasin, Anju/0000-0002-3687-8179; SANTORO, ROMUALDO/0000-0002-4360-4600; Scarlassara, Fernando/0000-0002-4663-8216; Turrisi, Rosario/0000-0002-5272-337X; Beole', Stefania/0000-0003-4673-8038; Barnby, Lee/0000-0001-7357-9904; Cosentino, Mauro/0000-0002-7880-8611; Bearden, Ian/0000-0003-2784-3094; Sumbera, Michal/0000-0002-0639-7323; Felea, Daniel/0000-0002-3734-9439; Peitzmann, Thomas/0000-0002-7116-899X; feofilov, grigory/0000-0003-3700-8623; Kovalenko, Vladimir/0000-0001-6012-6615; Castillo Castellanos, Javier/0000-0002-5187-2779; Takahashi, Jun/0000-0002-4091-1779; Guber, Fedor/0000-0001-8790-3218; Martinez Davalos, Arnulfo/0000-0002-9481-9548; Sevcenco, Adrian/0000-0002-4151-1056; Suaide, Alexandre/0000-0003-2847-6556; Deppman, Airton/0000-0001-9179-6363; Ferreiro, Elena/0000-0002-4449-2356; Armesto, Nestor/0000-0003-0940-0783; Ferretti, Alessandro/0000-0001-9084-5784; Martinez Hernandez, Mario Ivan/0000-0002-8503-3009; Vickovic, Linda/0000-0002-9820-7960; Fernandez Tellez, Arturo/0000-0003-0152-4220; Mohanty, Bedangadas/0000-0001-9610-2914; Vechernin, Vladimir/0000-0003-1458-8055; Janik, Malgorzata/0000-0002-3356-3438; Christensen, Christian/0000-0002-1850-0121; De Pasquale, Salvatore/0000-0001-9236-0748; Chinellato, David/0000-0002-9982-9577; de Cuveland, Jan/0000-0003-0455-1398; Kurepin, Alexey/0000-0002-1851-4136; Jena, Deepika/0000-0003-2112-0311; Akindinov, Alexander/0000-0002-7388-3022; Nattrass, Christine/0000-0002-8768-6468; Usai, Gianluca/0000-0002-8659-8378; Salgado, Carlos A./0000-0003-4586-2758; Bruna, Elena/0000-0001-5427-1461; Karasu Uysal, Ayben/0000-0001-6297-2532; Pshenichnov, Igor/0000-0003-1752-4524; Kompaniets, Mikhail/0000-0001-8831-0553; Altsybeev, Igor/0000-0002-8079-7026; Vinogradov, Leonid/0000-0001-9247-6230; Kondratiev, Valery/0000-0002-0031-0741 FU State Committee of Science; World Federation of Scientists (WFS); Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq); Financiadora de Estudos e Projetos (FINEP); Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC); Chinese Ministry of Education (CMOE); Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council; Carlsberg Foundation; Danish National Research Foundation; European Research Council under the European Community; Helsinki Institute of Physics; Academy of Finland; French CNRS-IN2P3; Region Pays de Loire; Region Alsace; Region Auvergne; CEA, France; German BMBF; Helmholtz Association; General Secretariat for Research and Technology, Ministry of Development, Greece; Hungarian OTKA; National Office for Research and Technology (NKTH); Department of Atomic Energy; Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN); Centro Fermi-Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi," Italy; MEXT, Japan; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); CONACYT; DGAPA, Mexico; ALFA-EC; HELEN Program (High-Energy physics Latin-American-European Network); Stichting voor Fundamenteel Onderzoek der Materie (FOM); Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); Polish Ministry of Science and Higher Education; National Authority for Scientific Research (NASR) (Autoritatea Nationala pentru Cercetare Stiintifica, ANCS); Ministry of Education and Science of Russian Federation; International Science and Technology Center; Russian Academy of Sciences; Russian Federal Agency of Atomic Energy; Russian Federal Agency for Science and Innovations; CERN-INTAS; Ministry of Education of Slovakia; Department of Science and Technology, South Africa; CIEMAT; EELA; Ministerio de Educacion y Ciencia of Spain; Xunta de Galicia (Conselleria de Educacion); CEADEN; Cubaenergia (Cuba); IAEA (International Atomic Energy Agency); Swedish Research Council (VR); Knut & Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); United States Department of Energy; United States National Science Foundation; State of Texas; State of Ohio FX We are grateful to P. Bozek, R. Fries, U. Heinz, Y. Karpenko, H. Petersen, J. Rafelski, C. Shen, Y. Sinyukov, H. Song, and K. Werner for providing the theoretical calculations and for the useful discussion and to colleagues from the BRAHMS, PHENIX, and STAR collaborations for the helpful discussions and clarifications on their measurements. The ALICE collaboration thanks all its engineers and technicians for their invaluable contributions to the construction of the experiment and the CERN accelerator teams for the outstanding performance of the LHC complex. The ALICE collaboration acknowledges the following funding agencies for their support in building and running the ALICE detector: the State Committee of Science, World Federation of Scientists (WFS) and Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq), Financiadora de Estudos e Projetos (FINEP), Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); the National Natural Science Foundation of China (NSFC), the Chinese Ministry of Education (CMOE), and the Ministry of Science and Technology of China (MSTC); the Ministry of Education and Youth of the Czech Republic; the Danish Natural Science Research Council, the Carlsberg Foundation, and the Danish National Research Foundation; The European Research Council under the European Community's Seventh Framework Programme; the Helsinki Institute of Physics and the Academy of Finland; French CNRS-IN2P3, the "Region Pays de Loire," "Region Alsace," "Region Auvergne," and CEA, France; German BMBF and the Helmholtz Association; the General Secretariat for Research and Technology, Ministry of Development, Greece; Hungarian OTKA and National Office for Research and Technology (NKTH); Department of Atomic Energy and Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN) and Centro Fermi-Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi," Italy; MEXT Grant-in-Aid for Specially Promoted Research, Japan; the Joint Institute for Nuclear Research, Dubna; the National Research Foundation of Korea (NRF); CONACYT, DGAPA, Mexico, ALFA-EC, and the HELEN Program (High-Energy physics Latin-American-European Network); the Stichting voor Fundamenteel Onderzoek der Materie (FOM) and the Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; the Research Council of Norway (NFR); the Polish Ministry of Science and Higher Education; the National Authority for Scientific Research (NASR) (Autoritatea Nationala pentru Cercetare Stiintifica, ANCS); the Ministry of Education and Science of Russian Federation, International Science and Technology Center, Russian Academy of Sciences, Russian Federal Agency of Atomic Energy, Russian Federal Agency for Science and Innovations, and CERN-INTAS; the Ministry of Education of Slovakia; the Department of Science and Technology, South Africa; CIEMAT, EELA, Ministerio de Educacion y Ciencia of Spain, Xunta de Galicia (Conselleria de Educacion), CEADEN, Cubaenergia (Cuba), and IAEA (International Atomic Energy Agency); the Swedish Research Council (VR) and Knut & Alice Wallenberg Foundation (KAW); the Ukraine Ministry of Education and Science; the United Kingdom Science and Technology Facilities Council (STFC); and the United States Department of Energy, the United States National Science Foundation, the State of Texas, and the State of Ohio. NR 70 TC 157 Z9 157 U1 8 U2 107 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD OCT 15 PY 2013 VL 88 IS 4 AR 044910 DI 10.1103/PhysRevC.88.044910 PG 23 WC Physics, Nuclear SC Physics GA 236UD UT WOS:000325824000005 ER PT J AU Abelev, B Adam, J Adamova, D Adare, AM Aggarwal, MM Rinella, GA Agnello, M Agocs, AG Agostinelli, A Ahammed, Z Ahmad, N Masoodi, AA Ahn, SU Ahn, SA Ajaz, M Akindinov, A Aleksandrov, D Alessandro, B Alici, A Alkin, A Avina, EA Alme, J Alt, T Altini, V Altinpinar, S Altsybeev, I Andrei, C Andronic, A Anguelov, V Anielski, J Anson, C Anticic, T Antinori, F Antonioli, P Aphecetche, L Appelshauser, H Arbor, N Arcelli, S Arend, A Armesto, N Arnaldi, R Aronsson, T Arsene, IC Arslandok, M Asryan, A Augustinus, A Averbeck, R Awes, TC Aysto, J Azmi, MD Bach, M Badala, A Baek, YW Bailhache, R Bala, R Baldisseri, A Pedrosa, FDS Ban, J Baral, RC Barbera, R Barile, F Barnafoldi, GG Barnby, LS Barret, V Bartke, J Basile, M Bastid, N Basu, S Bathen, B Batigne, G Batyunya, B Baumann, C Bearden, IG Beck, H Behera, NK Belikov, I Bellini, F Bellwied, R 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CA ALICE Collaboration TI Centrality determination of Pb-Pb collisions at root s(NN)=2.76 TeV with ALICE SO PHYSICAL REVIEW C LA English DT Article ID CROSS-SECTIONS; AA COLLISIONS; ENERGIES; PARTICLE; MODEL; PA; PP AB This publication describes the methods used to measure the centrality of inelastic Pb-Pb collisions at a center-of-mass energy of 2.76 TeV per colliding nucleon pair with ALICE. The centrality is a key parameter in the study of the properties of QCD matter at extreme temperature and energy density, because it is directly related to the initial overlap region of the colliding nuclei. Geometrical properties of the collision, such as the number of participating nucleons and the number of binary nucleon-nucleon collisions, are deduced from a Glauber model with a sharp impact parameter selection and shown to be consistent with those extracted from the data. 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H.; Viinikainen, J.] HIP, Jyvaskyla, Finland. [Aeystoe, J.; Chang, B.; Kalliokoski, T.; Kim, D. J.; Kral, J.; Krizek, F.; Loo, K. K.; Morreale, A.; Raiha, T. S.; Rak, J.; Rasanen, S. S.; Sarkamo, J.; Trzaska, W. H.; Viinikainen, J.] Univ Jyvaskyla, Jyvaskyla, Finland. [Azmi, M. D.; Bossu, F.; Buthelezi, Z.; Cleymans, J.; Fearick, R.; Foertsch, S.; Murray, S.; Steyn, G.; Vilakazi, Z.] Univ Cape Town, Dept Phys, Somerset West, South Africa. [Azmi, M. D.; Bossu, F.; Buthelezi, Z.; Cleymans, J.; Fearick, R.; Foertsch, S.; Murray, S.; Steyn, G.; Vilakazi, Z.] Natl Res Fdn, iThemba LABS, Somerset West, South Africa. [Badala, A.; Barbera, R.; Jacholkowski, A.; La Rocca, P.; Palmeri, A.; Pappalardo, G. S.; Petta, C.; Riggi, F.; Santagati, G.] Sezione Ist Nazl Fis Nucl, Catania, Italy. [Baek, Y. W.; Barret, V.; Bastid, N.; Crochet, P.; Dupieux, P.; Ichou, R.; Lopez, X.; Manso, F.; Marchisone, M.; Porteboeuf-Houssais, S.; Rosnet, P.; Vulpescu, B.; Zhang, X.] Univ Blaise Pascal, Clermont Univ, LPC, CNRS IN2P3, Clermont Ferrand, France. [Baek, Y. W.; Jung, H.; Kim, M.; Kim, J. S.; Kim, D. W.; Lee, K. S.; Lee, S. C.; Oh, S. K.] Gangneung Wonju Natl Univ, Kangnung, South Korea. [Bala, R.; Bhasin, A.; Gupta, R.; Gupta, A.; Mangotra, L.; Potukuchi, B.; Sambyal, S.; Sharma, S.; Rohni, S.; Singh, R.] Univ Jammu, Dept Phys, Jammu 180004, India. [Baldisseri, A.; Borel, H.; Castellanos, J. Castillo; Charvet, J. L.; Geuna, C.; Da Costa, H. Pereira; Rakotozafindrabe, A.; Yang, H.] IRFU, Comm Energie Atom, Saclay, France. [Ban, J.; Kalinak, P.; Kralik, I.; Krivda, M.; Mikhaylov, K.; Musinsky, J.; Pastircak, B.; Sandor, L.; Vala, M.] Slovak Acad Sci, Inst Expt Phys, Kosice 04353, Slovakia. [Baral, R. C.; Mahapatra, D. P.; Sahu, P. K.] Inst Phys, Bhubaneswar 751007, Orissa, India. [Barbera, R.; Jacholkowski, A.; La Rocca, P.; Petta, C.; Riggi, F.; Santagati, G.] Univ Catania, Dipartimento Fis & Astron, Catania, Italy. [Barnby, L. S.; Evans, D.; Hanratty, L. D.; Jones, P. G.; Jusko, A.; Krivda, M.; Lee, G. R.; Lietava, R.; Palaha, A.; Petrov, P.; Scott, P. A.; Baillie, O. Villalobos] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Bartke, J.; Figiel, J.; Gladysz-Dziadus, E.; Kowalski, M.; Matyja, A.; Mayer, C.; Rybicki, A.; Sputowska, I.; Szczepankiewicz, A.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Batyunya, B.; Grigoryan, S.; Malinina, L.; Mikhaylov, K.; Nomokonov, P.; Pocheptsov, T.; Rogochaya, E.; Shabratova, G.; Vala, M.; Vodopyanov, A.; Zaporozhets, S.] JINR, Dubna, Russia. [Bearden, I. G.; Bilandzic, A.; Boggild, H.; Chojnacki, M.; Christensen, C. H.; Gaardhoje, J. J.; Gulbrandsen, K.; Hansen, A.; Nielsen, B. S.; Nygaard, C.; Zaccolo, V.] Univ Copenhagen, Niels Bohr Inst, DK-2100 Copenhagen, Denmark. [Behera, N. K.; Dash, S.; Jena, S.; Meethaleveedu, G. Koyithatta; Kumar, J.; Nandi, B. K.; Nyatha, A.; Varma, R.] Indian Inst Technol Bombay IIT, Bombay, Maharashtra, India. [Belikov, I.; Hippolyte, B.; Kuhn, C.; Molnar, L.; Roy, C.; Castro, X. Sanchez; Senyukov, S.] Univ Strasbourg, IPHC, CNRS IN2P3, Strasbourg, France. [Bellwied, R.; Blanco, F.; Chinellato, D. D.; Jayarathna, P. H. S. Y.; Madagodahettige-Don, D. M.; Pinsky, L.; Piyarathna, D. B.; Timmins, A. R.; Weber, M.] Univ Houston, Houston, TX USA. [Beole, S.; Bianchi, L.; Botta, E.; Bruna, E.; Bufalino, S.; Morales, Y. Corrales; Ferretti, A.; Gagliardi, M.; Gallio, M.; Innocenti, G. M.; Marchisone, M.; Masera, M.; Milano, L.; Padilla, F.; Russo, R.; Vasquez, M. A. Subieta; Vercellin, E.] Univ Turin, Dipartimento Fis, Turin, Italy. [Berdnikov, Y.; Ivanov, V.; Khanzadeev, A.; Kryshen, E.; Malaev, M.; Nikulin, V.; Samsonov, V.; Zhalov, M.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Berzano, D.; Bhom, J.; Chujo, T.; Esumi, S.; Inaba, M.; Miake, Y.; Mizuno, S.; Niida, T.; Sakata, D.; Sano, M.; Watanabe, K.] Univ Tsukuba, Tsukuba, Ibaraki, Japan. [Bianchi, N.; Diaz, A. Casanova; Cunqueiro, L.; Di Nezza, P.; Fantoni, A.; Gianotti, P.; Muccifora, V.; Reolon, A. R.; Ronchetti, F.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Bjelogrlic, S.; de Rooij, R.; Dubla, A.; Grelli, A.; La Pointe, S. L.; Lodato, D. F.; Luparello, G.; Mischke, A.; Nooren, G.; Peitzmann, T.; Reicher, M.; Snellings, R. J. M.; Thomas, D.; van Leeuwen, M.; Veldhoen, M.; Verweij, M.; Yang, H.; Zhou, Y.] Univ Utrecht, Natl Inst Subat Phys, Nikhef, Utrecht, Netherlands. [Altini, V.; Bjelogrlic, S.; de Rooij, R.; Dubla, A.; Grelli, A.; La Pointe, S. L.; Lodato, D. F.; Luparello, G.; Mischke, A.; Nooren, G.; Peitzmann, T.; Reicher, M.; Snellings, R. J. M.; Thomas, D.; van Leeuwen, M.; Veldhoen, M.; Verweij, M.; Yang, H.; Zhou, Y.] Univ Utrecht, Inst Subat Phys, Utrecht, Netherlands. [Blanco, F.; Cotallo, M. E.; Corchero, M. A. Diaz; Gonzalez-Zamora, P.; Montes, E.; Rubio Montero, A. J.; Serradilla, E.] CIEMAT, Madrid, Spain. [Bottger, S.; Breitner, T.; Engel, H.; Kebschull, U.; Lara, C.; Ulrich, J.; Zelnicek, P.] Goethe Univ Frankfurt, Inst Informat, Frankfurt, Germany. [Bogdanov, A.; Grigoriev, V.; Kaplin, V.; Kondratyeva, N.; Loginov, V.] Moscow Engn Phys Inst, Moscow 115409, Russia. [Bogolyubsky, M.; Kharlov, Y.; Patalakha, D. I.; Polichtchouk, B.; Sadovsky, S.; Stolpovskiy, M.] Inst High Energy Phys, Protvino, Russia. [Altini, V.; Bombara, M.; Harmanova-Tothova, Z.; Kravcakova, A.; Putis, M.; Vrlakova, J.] Safarik Univ, Fac Sci, Kosice, Slovakia. [Altini, V.; Borissov, A.; Cormier, T. M.; Dobrin, A.; Jha, D. M.; Loggins, V. R.; Mlynarz, J.; Pavlinov, A.; Prasad, S. K.; Pruneau, C. A.; Putschke, J.; Voloshin, S.; Yaldo, C. G.] Wayne State Univ, Detroit, MI USA. [Botje, M.; Christakoglou, P.; Kuijer, P. G.; Lara, C. E. Perez; Manso, A. Rodriguez] NIKHEF H, Natl Inst Subat Phys, NL-1009 DB Amsterdam, Netherlands. [Braidot, E.; Cosentino, M. R.; Fenton-Olsen, B.; Jacobs, P. M.; Loizides, C.; Ploskon, M.; Rossi, A.; Sakai, S.; Symons, T. J. M.; Zhang, X.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Browning, T. A.; Scharenberg, R. P.; Srivastava, B. K.] Purdue Univ, W Lafayette, IN 47907 USA. [Broz, M.; Janik, R.; Meres, M.; Pikna, M.; Sitar, B.; Strmen, P.; Szarka, I.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Budnikov, D.; Filchagin, S.; Ilkaev, R.; Kuryakin, A.; Mamonov, A.; Nazarenko, S.; Punin, V.; Tumkin, A.; Vinogradov, Y.; Vyushin, A.; Zaviyalov, N.] Russian Fed Nucl Ctr VNIIEF, Sarov, Russia. [Caffarri, D.; Dainese, A.; Fabris, D.; Festanti, A.; Francescon, A.; Lunardon, M.; Morando, M.; Moretto, S.; Rossi, A.; Scarlassara, F.; Segato, G.; Soramel, F.; Toia, A.; Viesti, G.] Univ Padua, Dipartimento Fis & Astron, Padua, Italy. [Cai, X.; Li, S.; Luo, J.; Ma, K.; Mao, Y.; Wan, R.; Wang, Y.; Wang, M.; Wang, D.; Yin, Z.; Yuan, X.; Zhang, X.; Zhang, H.; Zhou, F.; Zhou, D.; Zhu, X.; Zhu, H.] Cent China Normal Univ, Wuhan, Peoples R China. [Villar, E. Calvo; Gago, A.] Pontificia Univ Catolica Peru, Dept Ciencias, Sec Fis, Lima, Peru. [Camerini, P.; Contin, G.; Lea, R.; Margagliotti, G. V.; Rui, R.; Venaruzzo, M.] Univ Trieste, Dipartmento Fis, I-34127 Trieste, Italy. [Camerini, P.; Contin, G.; Fragiacomo, E.; Grion, N.; Lea, R.; Margagliotti, G. V.; Piano, S.; Rachevski, A.; Rui, R.; Venaruzzo, M.] Sezione Ist Nazl Fis Nucl, Trieste, Italy. [Roman, V. Canoa; Contreras, J. G.; Crescio, E.; Albino, R. Cruz; Gomez, R.; Corral, G. Herrera; Montano Zetina, L.; Ramirez Reyes, A.] Ctr Invest Estudios Avanzados CINVESTAV, Mexico City, DF, Mexico. [Roman, V. Canoa; Contreras, J. G.; Crescio, E.; Albino, R. Cruz; Gomez, R.; Corral, G. Herrera; Montano Zetina, L.; Ramirez Reyes, A.] Ctr Invest Estudios Avanzados CINVESTAV, Merida, Mexico. [Agostinelli, A.; Carlin Filho, N.; de Barros, G. O. V.; Deppman, A.; Figueredo, M. A. S.; De Godoy, D. A. Moreira; Munhoz, M. G.; Da Silva, A. C. Oliveira; De Oliveira Filho, E. Pereira; Suaide, A. A. P.; de Toledo, A. Szanto] Univ Sao Paulo, Sao Paulo, Brazil. [Casula, E. A. R.; Collu, A.; De Falco, A.; Incani, E.; Puddu, G.; Serci, S.; Usai, G. L.] Univ Cagliari, Dipartimento Fis, Cagliari, Italy. [Casula, E. A. R.; Cicalo, C.; Collu, A.; De Falco, A.; Incani, E.; Masoni, A.; Puddu, G.; Serci, S.; Siddhanta, S.; Usai, G. L.] Sezione Ist Nazl Fis Nucl, Cagliari, Italy. [Sanchez, C. Ceballos; Lopez Torres, E.; Shtejer, K.] Ctr Aplicac Tecnol & Desarrollo Nucl CEADEN, Havana, Cuba. [Chang, B.; Kang, J. H.; Kim, M.; Kim, B.; Kim, T.; Kwon, Y.; Moon, T.; Song, M.; Yoon, J.] Yonsei Univ, Seoul 120749, South Korea. [Chattopadhyay, S.; Das, D.; Das, K.; Majumdar, A. K. Dutta; Khan, P.; Paul, B.; Roy, P.; Sinha, T.] Saha Inst Nucl Phys, Kolkata, India. [Cherney, M.; Nilsen, B. S.] Creighton Univ, Dept Phys, Omaha, NE 68178 USA. [Cheshkov, C.; Cheynis, B.; Ducroux, L.; Grossiord, J. -Y.; Guilbaud, M.; Tieulent, R.; Uras, A.; Zoccarato, Y.] Univ Lyon 1, CNRS IN2P3, IPN Lyon, F-69622 Villeurbanne, France. [Christiansen, P.; Dobrin, A.; Gros, P.; Ljunggren, H. M.; Ortiz Velasquez, A.; Oskarsson, A.; Richert, T.; Sogaard, C.; Stenlund, E.] Lund Univ, Div Expt High Energy Phys, Lund, Sweden. [Chung, S. U.; Seo, J.; Song, J.; Yi, J.; Yoo, I. -K.] Pusan Natl Univ, Pusan 609735, South Korea. [Cortese, P.; Ramello, L.; Sitta, M.] Univ Piemonte Orientale, Dipartimento Sci & Innovaz Tecnol, Alessandria, Italy. [Cortese, P.; Ramello, L.; Sitta, M.] Grp Collegato INFN, Alessandria, Italy. [Maldonado, I. Cortes; Tellez, A. Fernandez; Martinez, M. I.; Rodriguez Cahuantzi, M.; Tejeda Munoz, G.; Vargas, A.; Vergara, S.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Cuautle, E.; Jimenez Bustamante, R. T.; Ladron de Guevara, P.; Maldonado Cervantes, I.; Ortiz Velasquez, A.; Paic, G.; Simatovic, G.] Univ Nacl Autonoma Mexico, Inst Ciencias Nucl, Mexico City 04510, DF, Mexico. [Danu, A.; Felea, D.; Gheata, M.; Haiduc, M.; Mitu, C.; Niculescu, M.; Sevcenco, A.; Stan, I.; Zgura, I. S.] ISS, Bucharest, Romania. [Das, I.; Espagnon, B.; Hadjidakis, C.; Hrivnacova, I.; Lakomov, I.; Suire, C.; Takaki, J. D. Tapia; Palomo, L. Valencia] Univ Paris 11, IPNO, CNRS IN2P3, Orsay, France. [Das, S.] Bose Inst, Dept Phys, Kolkata, India. [Das, S.] CAPSS, Kolkata, India. [Dash, A.; Takahashi, J.] Univ Estadual Campinas UNICAMP, Campinas, SP, Brazil. [De Caro, A.; De Pasquale, S.; Girard, M. Fusco; Pagano, P.; Virgili, T.] Univ Salerno, Dipartimento Fis ER Caianiello, I-84100 Salerno, Italy. [De Caro, A.; De Pasquale, S.; Girard, M. Fusco; Pagano, P.; Virgili, T.] Grp Collegato INFN, Salerno, Italy. 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A.; Kisiel, A.; Oleniacz, J.; Ostrowski, P.; Pawlak, T.; Peryt, W.; Pluta, J.; Szymanski, M.; Zbroszczyk, H.] Warsaw Univ Technol, Warsaw, Poland. [Gomez, R.; Leon Monzon, I.; Podesta-Lerma, P. L. M.] Universidad Autonoma Sinaloa, Culiacan, Mexico. [Goswami, A.; Mishra, A. N.; Raniwala, S.; Raniwala, R.] Univ Rajasthan, Dept Phys, Jaipur 302004, Rajasthan, India. [Gotovac, S.; Mudnic, E.; Vickovic, L.] Tech Univ Split FESB, Split, Croatia. [Grigoryan, A.; Gulkanyan, H.; Hayrapetyan, A.; Papikyan, V.] Yerevan Phys Inst Fdn, AI Alikhanyan Natl Sci Lab, Yerevan, Armenia. [Gunji, T.; Hamagaki, H.; Hayashi, S.; Hori, Y.; Ozawa, K.; Torii, H.; Tsuji, T.; Yamaguchi, Y.] Univ Tokyo, Tokyo, Japan. [Han, B. H.; Hwang, D. S.; Kim, S.; Kim, J. H.; Son, H.] Sejong Univ, Dept Phys, Seoul, South Korea. [Hess, B. A.; Schmidt, H. R.; Wiechula, J.] Univ Tubingen, Tubingen, Germany. [Kalweit, A.; Mager, M.; Oeschler, H.] Tech Univ Darmstadt, Inst Kernphys, Darmstadt, Germany. [Uysal, A. Karasu] Yildiz Tech Univ, Istanbul, Turkey. [Uysal, A. Karasu] KTO Karatay Univ, Konya, Turkey. [Keidel, R.] Fachhochschule Worms, ZTT, Worms, Germany. [Klay, J. L.] Calif Polytech State Univ San Luis Obispo, San Luis Obispo, CA 93407 USA. [Knospe, A. G.; Markert, C.; Karampatsos, L. Xaplanteris] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Malinina, L.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Mares, J.; Polak, K.; Zavada, P.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Martashvili, I.; Mazer, J.; Nattrass, C.; Read, K. F.; Scott, R.; Sharma, N.] Univ Tennessee, Knoxville, TN USA. [Meddi, F.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Milosevic, J.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Milosevic, J.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Mishra, A. N.; Sahoo, R.] Indian Inst Technol Indore, Indore, India. [Mohanty, B.; Singha, S.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Pestov, Y.] Budker Inst Nucl Phys, Novosibirsk 630090, Russia. [Redlich, K.] Univ Wroclaw, Inst Theoret Phys, PL-50138 Wroclaw, Poland. [Ricci, R. A.; Vannucci, L.] Ist Nazl Fis Nucl, Lab Nazl Legnaro, I-35020 Legnaro, Italy. [Sakaguchi, H.; Shigaki, K.; Sugitate, T.] Hiroshima Univ, Hiroshima, Japan. [Ulrich, J.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Vernet, R.] Ctr Calcul IN2P3, Villeurbanne, France. RP Abelev, B (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RI Krizek, Filip/G-8967-2014; Bielcikova, Jana/G-9342-2014; Barnby, Lee/G-2135-2010; Blau, Dmitry/H-4523-2012; Yang, Hongyan/J-9826-2014; Cosentino, Mauro/L-2418-2014; Bearden, Ian/M-4504-2014; Sumbera, Michal/O-7497-2014; Felea, Daniel/C-1885-2012; Barnafoldi, Gergely Gabor/L-3486-2013; Peitzmann, Thomas/K-2206-2012; Kharlov, Yuri/D-2700-2015; Kovalenko, Vladimir/C-5709-2013; feofilov, grigory/A-2549-2013; Castillo Castellanos, Javier/G-8915-2013; Martinez Davalos, Arnulfo/F-3498-2013; Bregant, Marco/I-7663-2012; Levai, Peter/A-1544-2014; Pochybova, Sona/A-2835-2014; Takahashi, Jun/B-2946-2012; Wagner, Vladimir/G-5650-2014; Sevcenco, Adrian/C-1832-2012; Vajzer, Michal/G-8469-2014; Guber, Fedor/I-4271-2013; Akindinov, Alexander/J-2674-2016; Nattrass, Christine/J-6752-2016; Suaide, Alexandre/L-6239-2016; Deppman, Airton/J-5787-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Ferreiro, Elena/C-3797-2017; Armesto, Nestor/C-4341-2017; Ferretti, Alessandro/F-4856-2013; Martinez Hernandez, Mario Ivan/F-4083-2010; Vickovic, Linda/F-3517-2017; Fernandez Tellez, Arturo/E-9700-2017; Vechernin, Vladimir/J-5832-2013; Graczykowski, Lukasz/O-7522-2015; Janik, Malgorzata/O-7520-2015; Adamova, Dagmar/G-9789-2014; Christensen, Christian/D-6461-2012; De Pasquale, Salvatore/B-9165-2008; Chinellato, David/D-3092-2012; de Cuveland, Jan/H-6454-2016; Kurepin, Alexey/H-4852-2013; Jena, Deepika/P-2873-2015; Jena, Satyajit/P-2409-2015; Mitu, Ciprian/E-6733-2011; Usai, Gianluca/E-9604-2015; Salgado, Carlos A./G-2168-2015; Bruna, Elena/C-4939-2014; Karasu Uysal, Ayben/K-3981-2015; HAMAGAKI, HIDEKI/G-4899-2014; Pshenichnov, Igor/A-4063-2008; Kompaniets, Mikhail/F-5025-2013; Altsybeev, Igor/K-6687-2013; Vinogradov, Leonid/K-3047-2013; Kondratiev, Valery/J-8574-2013 OI Barnby, Lee/0000-0001-7357-9904; Cosentino, Mauro/0000-0002-7880-8611; Bearden, Ian/0000-0003-2784-3094; Sumbera, Michal/0000-0002-0639-7323; Felea, Daniel/0000-0002-3734-9439; Peitzmann, Thomas/0000-0002-7116-899X; Kovalenko, Vladimir/0000-0001-6012-6615; feofilov, grigory/0000-0003-3700-8623; Castillo Castellanos, Javier/0000-0002-5187-2779; Martinez Davalos, Arnulfo/0000-0002-9481-9548; Takahashi, Jun/0000-0002-4091-1779; Sevcenco, Adrian/0000-0002-4151-1056; Guber, Fedor/0000-0001-8790-3218; Beole', Stefania/0000-0003-4673-8038; Mohanty, Bedangadas/0000-0001-9610-2914; Gago Medina, Alberto Martin/0000-0002-0019-9692; Dainese, Andrea/0000-0002-2166-1874; Paticchio, Vincenzo/0000-0002-2916-1671; Monteno, Marco/0000-0002-3521-6333; Bhasin, Anju/0000-0002-3687-8179; SANTORO, ROMUALDO/0000-0002-4360-4600; Scarlassara, Fernando/0000-0002-4663-8216; Turrisi, Rosario/0000-0002-5272-337X; Akindinov, Alexander/0000-0002-7388-3022; Nattrass, Christine/0000-0002-8768-6468; Suaide, Alexandre/0000-0003-2847-6556; Deppman, Airton/0000-0001-9179-6363; Ferreiro, Elena/0000-0002-4449-2356; Armesto, Nestor/0000-0003-0940-0783; Ferretti, Alessandro/0000-0001-9084-5784; Martinez Hernandez, Mario Ivan/0000-0002-8503-3009; Vickovic, Linda/0000-0002-9820-7960; Fernandez Tellez, Arturo/0000-0003-0152-4220; Vechernin, Vladimir/0000-0003-1458-8055; Janik, Malgorzata/0000-0002-3356-3438; Christensen, Christian/0000-0002-1850-0121; De Pasquale, Salvatore/0000-0001-9236-0748; Chinellato, David/0000-0002-9982-9577; de Cuveland, Jan/0000-0003-0455-1398; Kurepin, Alexey/0000-0002-1851-4136; Jena, Deepika/0000-0003-2112-0311; Jena, Satyajit/0000-0002-6220-6982; Usai, Gianluca/0000-0002-8659-8378; Salgado, Carlos A./0000-0003-4586-2758; Bruna, Elena/0000-0001-5427-1461; Karasu Uysal, Ayben/0000-0001-6297-2532; Pshenichnov, Igor/0000-0003-1752-4524; Kompaniets, Mikhail/0000-0001-8831-0553; Altsybeev, Igor/0000-0002-8079-7026; Vinogradov, Leonid/0000-0001-9247-6230; Kondratiev, Valery/0000-0002-0031-0741 FU State Committee of Science; Calouste Gulbenkian Foundation from Lisbon; Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq); Financiadora de Estudos e Projetos (FINEP); Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC); Chinese Ministry of Education (CMOE); Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council; Carlsberg Foundation; Danish National Research Foundation; European Research Council under the European Community; Helsinki Institute of Physics; Academy of Finland; French CNRS-IN2P3; Region Pays de Loire; Region Alsace; Region Auvergne; CEA, France; German BMBF; Helmholtz Association; General Secretariat for Research and Technology, Ministry of Development, Greece; Hungarian OTKA; National Office for Research and Technology (NKTH); Department of Atomic Energy; Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN); Centro Fermi, Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi," Italy; MEXT, Japan; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); CONACYT; DGAPA, Mexico; ALFA-EC; HELEN Program (High-Energy physics Latin-American-European Network); Stichting voor Fundamenteel Onderzoek der Materie (FOM); Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); Polish Ministry of Science and Higher Education; National Authority for Scientific Research (NASR) (Autoritatea Nationala pentru Cercetare Stiintifica, ANCS); Ministry of Education and Science of Russian Federation; International Science and Technology Center, Russian Academy of Sciences; Russian Federal Agency of Atomic Energy; Russian Federal Agency for Science and Innovations and CERN-INTAS; Ministry of Education of Slovakia; Department of Science and Technology, South Africa; CIEMAT; EELA; Ministerio de Educacion y Ciencia of Spain; Xunta de Galicia (Conselleria de Educacion); CEADEN; Cubaenergia (Cuba); IAEA (International Atomic Energy Agency); Swedish Research Council (VR); Knut & Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); United States Department of Energy; United States National Science Foundation; State of Texas; State of Ohio FX The ALICE collaboration thanks all its engineers and technicians for their invaluable contributions to the construction of the experiment and the CERN accelerator teams for the outstanding performance of the LHC complex. The ALICE collaboration acknowledges the following funding agencies for their support in building and running the ALICE detector: State Committee of Science, Calouste Gulbenkian Foundation from Lisbon and Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq), Financiadora de Estudos e Projetos (FINEP), and Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); the National Natural Science Foundation of China (NSFC), the Chinese Ministry of Education (CMOE), and the Ministry of Science and Technology of China (MSTC); the Ministry of Education and Youth of the Czech Republic; the Danish Natural Science Research Council, the Carlsberg Foundation, and the Danish National Research Foundation; The European Research Council under the European Community's Seventh Framework Programme; the Helsinki Institute of Physics and the Academy of Finland; French CNRS-IN2P3, the "Region Pays de Loire," "Region Alsace," "Region Auvergne" and CEA, France; German BMBF and the Helmholtz Association; the General Secretariat for Research and Technology, Ministry of Development, Greece; the Hungarian OTKA and National Office for Research and Technology (NKTH); the Department of Atomic Energy and Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN) and Centro Fermi, Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi," Italy; MEXT Grant-in-Aid for Specially Promoted Research, Japan; the Joint Institute for Nuclear Research, Dubna; the National Research Foundation of Korea (NRF); CONACYT, DGAPA, Mexico, ALFA-EC, and the HELEN Program (High-Energy physics Latin-American-European Network); Stichting voor Fundamenteel Onderzoek der Materie (FOM) and the Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; the Research Council of Norway (NFR); the Polish Ministry of Science and Higher Education; the National Authority for Scientific Research (NASR) (Autoritatea Nationala pentru Cercetare Stiintifica, ANCS); Ministry of Education and Science of Russian Federation, International Science and Technology Center, Russian Academy of Sciences, Russian Federal Agency of Atomic Energy, Russian Federal Agency for Science and Innovations and CERN-INTAS; the Ministry of Education of Slovakia; the Department of Science and Technology, South Africa; CIEMAT, EELA, Ministerio de Educacion y Ciencia of Spain, Xunta de Galicia (Conselleria de Educacion), CEADEN, Cubaenergia (Cuba), and IAEA (International Atomic Energy Agency); the Swedish Research Council (VR) and Knut & Alice Wallenberg Foundation (KAW); the Ukraine Ministry of Education and Science; the United Kingdom Science and Technology Facilities Council (STFC); the United States Department of Energy, the United States National Science Foundation, the State of Texas, and the State of Ohio. NR 46 TC 105 Z9 105 U1 5 U2 96 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD OCT 15 PY 2013 VL 88 IS 4 AR 044909 DI 10.1103/PhysRevC.88.044909 PG 22 WC Physics, Nuclear SC Physics GA 236UD UT WOS:000325824000004 ER PT J AU Hoffman, CR Albers, M Alcorta, M Almaraz-Calderon, S Back, BB Baker, SI Bedoor, S Bertone, PF Kay, BP Lighthall, JC Palchan, T Pardo, RC Perdikakis, G Rehm, KE Rogers, AM Santiago-Gonzalez, D Yuan, C Schiffer, JP AF Hoffman, C. R. Albers, M. Alcorta, M. Almaraz-Calderon, S. Back, B. B. Baker, S. I. Bedoor, S. Bertone, P. F. Kay, B. P. Lighthall, J. C. Palchan, T. Pardo, R. C. Perdikakis, G. Rehm, K. E. Rogers, A. M. Santiago-Gonzalez, D. Yuan, Cenxi Schiffer, J. P. TI Single-neutron excitations in N-18 SO PHYSICAL REVIEW C LA English DT Article ID EXCITED-STATES; ENERGY-LEVELS; LIGHT-NUCLEI; GROUND-STATE; BETA-DECAY; MAGNETIC-MOMENT; SHELL-MODEL; C-17; MASS; C-17,C-19 AB States in N-18 have been populated in the neutron-adding (d, p) reaction on the short-lived N-17 beam. Previously observed levels, found in this work at excitation energies of 0.12(1) MeV and 0.74(1) MeV, have been identified as those expected from a proton 0p(1/2) hole coupled to the O-19 5/2(+) ground state. A new state at 1.17(2) MeV is consistent with the coupling of the 1/2(-) proton-hole state to the excited 1/2(+) state in O-19. Orbital angular momentum assignments and spectroscopic factors were determined from the measured angular distributions through a distorted wave Born approximation analysis. Systematics for the (0d(5/2)1s(1/2))(3) neutron configurations in the N = 11 isotones, C-17, N-18, and O-19 are discussed and comparisons to p-sd shell-model calculations are made. C1 [Hoffman, C. R.; Albers, M.; Alcorta, M.; Almaraz-Calderon, S.; Back, B. B.; Baker, S. I.; Bertone, P. F.; Kay, B. P.; Lighthall, J. C.; Palchan, T.; Pardo, R. C.; Rehm, K. E.; Rogers, A. M.; Schiffer, J. P.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Bedoor, S.; Lighthall, J. C.] Western Michigan Univ, Dept Phys, Kalamazoo, MI 49008 USA. [Kay, B. P.] Univ York, Dept Phys, York YO10 5DD, N Yorkshire, England. [Perdikakis, G.] Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA. [Perdikakis, G.] Cent Michigan Univ, Dept Phys, Mt Pleasant, MI 48859 USA. [Santiago-Gonzalez, D.] Florida State Univ, Dept Phys, Tallahassee, FL 32306 USA. [Yuan, Cenxi] Sun Yat Sen Univ, Sino French Inst Nucl Engn & Technol, Zhuhai 519082, Peoples R China. RP Hoffman, CR (reprint author), Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. EM calem.hoffman@gmail.com RI Alcorta, Martin/G-7107-2011; Yuan, Cenxi/A-5115-2013; Perdikakis, Georgios/K-4525-2014; Hoffman, Calem/H-4325-2016 OI Alcorta, Martin/0000-0002-6217-5004; Yuan, Cenxi/0000-0002-3495-3614; Perdikakis, Georgios/0000-0002-8539-8737; Hoffman, Calem/0000-0001-7141-9827 FU U.S. Department of Energy, Office of Nuclear Physics [DE-AC02-06CH11357, DE-FG02-04ER41320]; National Science Foundation [PHY-10-64819, PHY-11-02511]; UK Science and Technology Facilities Council FX The authors would like to acknowledge the hard work of the support and operations staff at ATLAS. Thanks to J. P. Greene for preparations of all targets. This work was supported by the U.S. Department of Energy, Office of Nuclear Physics, under Contract No. DE-AC02-06CH11357 (ANL) and Grant No. DE-FG02-04ER41320 (WMU); also, by the National Science Foundation under Grants No. PHY-10-64819 (FSU) and No. PHY-11-02511 (NSCL), and by a grant from the UK Science and Technology Facilities Council. NR 56 TC 1 Z9 1 U1 1 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD OCT 15 PY 2013 VL 88 IS 4 AR 044317 DI 10.1103/PhysRevC.88.044317 PG 7 WC Physics, Nuclear SC Physics GA 236UD UT WOS:000325824000001 ER PT J AU Deshpande, R Asiedu, MK Klebig, M Sutor, S Kuzmin, E Nelson, J Piotrowski, J Shin, SH Yoshida, M Costanzo, M Boone, C Wigle, DA Myers, CL AF Deshpande, Raamesh Asiedu, Michael K. Klebig, Mitchell Sutor, Shari Kuzmin, Elena Nelson, Justin Piotrowski, Jeff Shin, Seung Ho Yoshida, Minoru Costanzo, Michael Boone, Charles Wigle, Dennis A. Myers, Chad L. TI A Comparative Genomic Approach for Identifying Synthetic Lethal Interactions in Human Cancer SO CANCER RESEARCH LA English DT Article ID SOFT-PART SARCOMA; POLY(ADP-RIBOSE) POLYMERASE; RNA INTERFERENCE; OVARIAN-CANCER; CELL-LINES; TUMORS; GENE; VULNERABILITIES; DISCOVERY; REVEALS AB Synthetic lethal interactions enable a novel approach for discovering specific genetic vulnerabilities in cancer cells that can be exploited for the development of therapeutics. Despite successes in model organisms such as yeast, discovering synthetic lethal interactions on a large scale in human cells remains a significant challenge. We describe a comparative genomic strategy for identifying cancer-relevant synthetic lethal interactions whereby candidate interactions are prioritized on the basis of genetic interaction data available in yeast, followed by targeted testing of candidate interactions in human cell lines. As a proof of principle, we describe two novel synthetic lethal interactions in human cells discovered by this approach, one between the tumor suppressor gene SMARCB1 and PSMA4, and another between alveolar soft-part sarcoma-associated ASPSCR1 and PSMC2. These results suggest therapeutic targets for cancers harboring mutations in SMARCB1 or ASPSCR1 and highlight the potential of a targeted, cross-species strategy for identifying synthetic lethal interactions relevant to human cancer. Cancer Res; 73(20); 6128-36. (C) 2013 AACR. C1 [Deshpande, Raamesh; Myers, Chad L.] Univ Minnesota, Dept Comp Sci & Engn, Minneapolis, MN USA. [Nelson, Justin; Shin, Seung Ho; Wigle, Dennis A.; Myers, Chad L.] Univ Minnesota, Program Biomed Informat & Computat Biol, Minneapolis, MN USA. [Asiedu, Michael K.; Klebig, Mitchell; Sutor, Shari; Wigle, Dennis A.] Mayo Clin, Dept Surg, Rochester, MN USA. [Klebig, Mitchell] Mayo Clin, Dept Lab Med & Pathol, Mol Genet Lab, Rochester, MN USA. [Kuzmin, Elena; Costanzo, Michael; Boone, Charles] Univ Toronto, Terrence Donnelly Ctr Cellular & Biomol Res, Dept Mol Genet, Toronto, ON M5S 1A1, Canada. [Yoshida, Minoru; Boone, Charles] RIKEN, Adv Sci Inst, Chem Genom Res Grp, Saitama, Japan. [Piotrowski, Jeff] Univ Wisconsin, Great Lakes Bioenergy Res Ctr, Madison, WI USA. RP Myers, CL (reprint author), Univ Minnesota Twin Cities, 200 Union St SE, Minneapolis, MN 55455 USA. EM wigle.dennis@mayo.edu; cmyers@cs.umn.edu RI Yoshida, Minoru/C-8049-2014 FU Minnesota Partnership for Biotechnology and Medical Genomics program; University of Minnesota Doctoral Dissertation Fellowship; Biomedical Informatics and Computational Biology (BICB) traineeship; NIH [1R01HG005084-01A1, 1R01HG005853-01]; National Science Foundation [DBI 0953881]; Canadian Institutes of Health Research [MOP-102629, MOP-97939, MOP-57830]; Ontario Research Fund [GL2-01-22]; BICB fellowship; RIKEN President's Discretionary Fund; Canadian Institute for Advanced Research (CIFAR) Genetic Networks Program FX This work was financially supported by a grant from the Minnesota Partnership for Biotechnology and Medical Genomics program to C.L. Myers and D.A. Wigle. R. Deshpande was funded by a University of Minnesota Doctoral Dissertation Fellowship and Biomedical Informatics and Computational Biology (BICB) traineeship. C.L. Myers and R. Deshpande are also partially supported by a grant from the NIH (1R01HG005084-01A1) and a grant from the National Science Foundation (DBI 0953881). C. Boone is supported by the Canadian Institutes of Health Research (grant nos. MOP-102629, MOP-97939, and MOP-57830), the Ontario Research Fund (grant no. GL2-01-22), and the NIH (grant no. 1R01HG005853-01). S.H. Shin was supported by a BICB fellowship. C. Boone, M. Yoshida, and J. Piotrowski are supported by the RIKEN President's Discretionary Fund. C.L. Myers and C. Boone are partially supported by the Canadian Institute for Advanced Research (CIFAR) Genetic Networks Program. NR 31 TC 13 Z9 13 U1 2 U2 13 PU AMER ASSOC CANCER RESEARCH PI PHILADELPHIA PA 615 CHESTNUT ST, 17TH FLOOR, PHILADELPHIA, PA 19106-4404 USA SN 0008-5472 EI 1538-7445 J9 CANCER RES JI Cancer Res. PD OCT 15 PY 2013 VL 73 IS 20 BP 6128 EP 6136 DI 10.1158/0008-5472.CAN-12-3956 PG 9 WC Oncology SC Oncology GA 236KV UT WOS:000325796100006 PM 23980094 ER PT J AU Jackson, GS Hillegonds, DJ Muzikar, P Goehring, B AF Jackson, George S. Hillegonds, Darren J. Muzikar, Paul Goehring, Brent TI Ultra-trace analysis of Ca-41 in urine by accelerator mass spectrometry: An inter-laboratory comparison SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS LA English DT Article DE Ca-41; Accelerator mass spectrometry; Bayesian statistics; Interlaboratory comparison ID POSTMENOPAUSAL WOMEN; CALCIUM-METABOLISM; BONE-RESORPTION; AMS AB A Ca-41 interlaboratory comparison between Lawrence Livermore National Laboratory (LLNL) and the Purdue Rare Isotope Laboratory (PRIME Lab) has been completed. Analysis of the ratios assayed by accelerator mass spectrometry (AMS) shows that there is no statistically significant difference in the ratios. Further, Bayesian analysis shows that the uncertainties reported by both facilities are correct with the possibility of a slight under-estimation by one laboratory. Finally, the chemistry procedures used by the two facilities to produce CaF2 for the cesium sputter ion source are robust and do not yield any significant differences in the final result. (C) 2013 Elsevier B.V. All rights reserved. C1 [Jackson, George S.; Muzikar, Paul; Goehring, Brent] Purdue Univ, PRIME Lab, W Lafayette, IN 47907 USA. [Hillegonds, Darren J.] Lawrence Livermore Natl Lab, Div Chem Sci, Livermore, CA 94550 USA. [Hillegonds, Darren J.] Lawrence Livermore Natl Lab, Ctr Accelerator Mass Spectrometry, Livermore, CA 94550 USA. RP Jackson, GS (reprint author), Purdue Univ, Purdue Rare Isotope Measurement Lab, 525 Northwestern Ave, W Lafayette, IN 47907 USA. EM jacksogs@purdue.edu FU National Institutes of Health [P50-AT00477, R21-CA127671]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was supported by grants P50-AT00477 and R21-CA127671 from the National Institutes of Health. LLNL efforts were performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 27 TC 4 Z9 4 U1 0 U2 9 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-583X EI 1872-9584 J9 NUCL INSTRUM METH B JI Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms PD OCT 15 PY 2013 VL 313 BP 14 EP 20 DI 10.1016/j.nimb.2013.08.004 PG 7 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 231WG UT WOS:000325448500003 ER PT J AU DeMaere, MZ Williams, TJ Allen, MA Brown, MV Gibson, JAE Rich, J Lauro, FM Dyall-Smith, M Davenport, KW Woyke, T Kyrpides, NC Tringe, SG Cavicchioli, R AF DeMaere, Matthew Z. Williams, Timothy J. Allen, Michelle A. Brown, Mark V. Gibson, John A. E. Rich, John Lauro, Federico M. Dyall-Smith, Michael Davenport, Karen W. Woyke, Tanja Kyrpides, Nikos C. Tringe, Susannah G. Cavicchioli, Ricardo TI High level of intergenera gene exchange shapes the evolution of haloarchaea in an isolated Antarctic lake SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE mobile genetic elements; Antarctic haloarchaea; saltern; fragment recruitment; BJ1 virus ID VESTFOLD HILLS; DEEP LAKE; EAST ANTARCTICA; SALINE LAKES; HYPERSALINE; ARCHAEA; GENOMICS; SEQUENCE; SALTERN; RECOMBINATION AB Deep Lake in Antarctica is a globally isolated, hypersaline system that remains liquid at temperatures down to -20 degrees C. By analyzing metagenome data and genomes of four isolates we assessed genome variation and patterns of gene exchange to learn how the lake community evolved. The lake is completely and uniformly dominated by haloarchaea, comprising a hierarchically structured, low-complexity community that differs greatly to temperate and tropical hypersaline environments. The four Deep Lake isolates represent distinct genera (similar to 85% 16S rRNA gene similarity and similar to 73% genome average nucleotide identity) with genomic characteristics indicative of niche adaptation, and collectively account for similar to 72% of the cellular community. Network analysis revealed a remarkable level of intergenera gene exchange, including the sharing of long contiguous regions (up to 35 kb) of high identity (similar to 100%). Although the genomes of closely related Halobacterium, Haloquadratum, and Haloarcula (>90% average nucleotide identity) shared regions of high identity between species or strains, the four Deep Lake isolates were the only distantly related haloarchaea to share long high-identity regions. Moreover, the Deep Lake high-identity regions did not match to any other hypersaline environment metagenome data. The most abundant species, tADL, appears to play a central role in the exchange of insertion sequences, but not the exchange of high-identity regions. The genomic characteristics of the four haloarchaea are consistent with a lake ecosystem that sustains a high level of intergenera gene exchange while selecting for ecotypes that maintain sympatric speciation. The peculiarities of this polar system restrict which species can grow and provide a tempo and mode for accentuating gene exchange. C1 [DeMaere, Matthew Z.; Williams, Timothy J.; Allen, Michelle A.; Brown, Mark V.; Rich, John; Lauro, Federico M.; Cavicchioli, Ricardo] Univ New S Wales, Sch Biotechnol & Biomol Sci, Sydney, NSW 2052, Australia. [Brown, Mark V.] Univ New S Wales, Evolut & Ecol Res Ctr, Sydney, NSW 2052, Australia. [Gibson, John A. E.] Univ Tasmania, Inst Marine & Antarctic Studies, Hobart, Tas 7001, Australia. [Dyall-Smith, Michael] Charles Sturt Univ, Wagga Wagga, NSW 2678, Australia. [Davenport, Karen W.] Los Alamos Natl Lab, Dept Energy Joint Genome Inst, Biosci Div, Los Alamos, NM 87545 USA. [Woyke, Tanja; Kyrpides, Nikos C.; Tringe, Susannah G.] Dept Energy Joint Genome Inst, Walnut Creek, CA 94598 USA. RP Cavicchioli, R (reprint author), Univ New S Wales, Sch Biotechnol & Biomol Sci, Sydney, NSW 2052, Australia. EM r.cavicchioli@unsw.edu.au RI Kyrpides, Nikos/A-6305-2014; OI Kyrpides, Nikos/0000-0002-6131-0462; Lauro, Federico/0000-0002-8373-1014; DeMaere, Matthew/0000-0002-7601-5108 FU Australian Research Council; Australian Antarctic Science program; Australian Government; Office of Science of the US DOE [DE-AC02-05CH11231]; Max Planck Society FX We thank Nico Wanandy for extracting DNA from filters, Yan Liao for assistance with PCR and sequencing of HIR, Aaron Darling for helpful discussions, Philip Johnson for guidance on the use of Population genetic Inference In Metagenomics, Jon Magnuson and Jerry Jenkins for access to the draft Dunaliella salina Culture Collection of Algae and Protozoa 19/18 genome sequence, and Tassia Kolesnikow for comments on the manuscript. We also thank the Editor and reviewers who provided very insightful and constructive feedback. This work was supported by the Australian Research Council and the Australian Antarctic Science program and undertaken with the assistance of resources provided at the National Computational Infrastructure National Facility systems at the Australian National University through the National Computational Merit Allocation Scheme supported by the Australian Government. The work conducted by the US DOE Joint Genome Institute is supported by the Office of Science of the US DOE under Contract DE-AC02-05CH11231. M.D.S. is grateful for the support by the Max Planck Society, and particularly D. Oesterhelt (Department of Membrane Biochemistry, Max Planck Institute). NR 49 TC 38 Z9 41 U1 7 U2 49 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD OCT 15 PY 2013 VL 110 IS 42 BP 16939 EP 16944 DI 10.1073/pnas.1307090110 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 234HT UT WOS:000325634200056 PM 24082106 ER PT J AU Ortmann, JE Liu, JY Hu, J Zhu, M Peng, J Matsuda, M Ke, X Mao, ZQ AF Ortmann, J. E. Liu, J. Y. Hu, J. Zhu, M. Peng, J. Matsuda, M. Ke, X. Mao, Z. Q. TI Competition Between Antiferromagnetism and Ferromagnetism in Sr2RuO4 Probed by Mn and Co Doping SO SCIENTIFIC REPORTS LA English DT Article ID SPIN-TRIPLET SUPERCONDUCTIVITY; UNCONVENTIONAL SUPERCONDUCTIVITY; DEPENDENCE; CRYSTAL; NMR AB Spin-triplet superconductivity in Sr2RuO4 has attracted enormous interest. Like other unconventional superconductors, superconductivity in Sr2RuO4 is in close proximity to magnetic instability. Undoped Sr2RuO4 exhibits incommensurate antiferromagnetic (AFM) fluctuations, which can evolve into static, short-range AFM order via Ti doping. Moreover, weak ferromagnetic (FM) coupling in Sr2RuO4 has also been suggested by NMR/neutron scattering experiments and studies on Ca2-xSrxRuO4 and Sr2-yLayRuO4, implying orbital dependent magnetism. We report bulk static, short-range FM order in Sr2RuO4 triggered by <2% Co doping, showing superconductivity in Sr2RuO4 is much closer to FM instability than previously reported in Ca2-xSrxRuO4. We also find Mn doping can effectively establish incommensurate AFM order, with T-N similar to 50 K for 3% Mn doping. These new results place Sr2RuO4 in a unique situation where superconductivity lies directly on the borderline of two distinct magnetic states, highlighting the important role of competing magnetic fluctuations in determining superconducting properties of Sr2RuO4. C1 [Ortmann, J. E.; Liu, J. Y.; Hu, J.; Peng, J.; Mao, Z. Q.] Tulane Univ, Dept Phys & Engn Phys, New Orleans, LA 70118 USA. [Zhu, M.; Ke, X.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Matsuda, M.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. RP Mao, ZQ (reprint author), Tulane Univ, Dept Phys & Engn Phys, New Orleans, LA 70118 USA. EM zmao@tulane.edu RI Hu, Jin/C-4141-2014; Matsuda, Masaaki/A-6902-2016 OI Hu, Jin/0000-0003-0080-4239; Matsuda, Masaaki/0000-0003-2209-9526 FU NSF [DMR-1205469]; LA-SiGMA program [EPS-1003897]; Michigan State University; DOE basic Energy Sciences, Scientific User Facilities Division FX The work is supported by the NSF under grant DMR-1205469 and the LA-SiGMA program under award #EPS-1003897. X. K. acknowledges the financial support from the start-up funds at Michigan State University. Research at ORNL's High Flux Isotope Reactor was sponsored by DOE basic Energy Sciences, Scientific User Facilities Division. The authors are grateful to L. Zheng and X.S. Wu for informative discussions. NR 42 TC 16 Z9 16 U1 5 U2 50 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD OCT 15 PY 2013 VL 3 AR 2950 DI 10.1038/srep02950 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 233ZQ UT WOS:000325608800011 PM 24126684 ER PT J AU Curtis, DS Phillips, AR Callister, SJ Conlan, S McCue, LA AF Curtis, Darren S. Phillips, Aaron R. Callister, Stephen J. Conlan, Sean McCue, Lee Ann TI SPOCS: software for predicting and visualizing orthology/paralogy relationships among genomes SO BIOINFORMATICS LA English DT Article AB At the rate that prokaryotic genomes can now be generated, comparative genomics studies require a flexible method for quickly and accurately predicting orthologs among the rapidly changing set of genomes available. SPOCS implements a graph-based ortholog prediction method to generate a simple tab-delimited table of orthologs and in addition, html files that provide a visualization of the predicted ortholog/paralog relationships to which gene/protein expression metadata may be overlaid. C1 [Curtis, Darren S.; Phillips, Aaron R.] Pacific NW Natl Lab, Computat & Stat Analyt Div, Richland, WA 99352 USA. [Callister, Stephen J.] Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99352 USA. [Conlan, Sean] NHGRI, Genet & Mol Biol Branch, NIH, Bethesda, MD 20892 USA. [McCue, Lee Ann] Pacific NW Natl Lab, Computat Sci & Math Div, Richland, WA 99352 USA. RP McCue, LA (reprint author), Pacific NW Natl Lab, Computat Sci & Math Div, Richland, WA 99352 USA. EM leeann.mccue@pnnl.gov RI Conlan, Sean/B-4401-2008; OI Conlan, Sean/0000-0001-6848-3465; Curtis, Darren/0000-0002-4907-4575; McCue, Lee Ann/0000-0003-4456-517X FU U.S. Department of Energy, Office of Biological and Environmental Research (DOE-BER) Genome Science Program; DOE [DE-AC06-76RL01830] FX This work was supported by U.S. Department of Energy, Office of Biological and Environmental Research (DOE-BER) Genome Science Program, and performed at the Pacific Northwest National Laboratory, a multiprogram national laboratory operated by Battelle for the DOE under Contract DE-AC06-76RL01830. NR 7 TC 5 Z9 5 U1 0 U2 9 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 1367-4803 J9 BIOINFORMATICS JI Bioinformatics PD OCT 15 PY 2013 VL 29 IS 20 BP 2641 EP 2642 DI 10.1093/bioinformatics/btt454 PG 2 WC Biochemical Research Methods; Biotechnology & Applied Microbiology; Computer Science, Interdisciplinary Applications; Mathematical & Computational Biology; Statistics & Probability SC Biochemistry & Molecular Biology; Biotechnology & Applied Microbiology; Computer Science; Mathematical & Computational Biology; Mathematics GA 232ID UT WOS:000325485800017 PM 23956303 ER PT J AU Cismasu, AC Levard, C Michel, FM Brown, GE AF Cismasu, A. Cristina Levard, Clement Michel, F. Marc Brown, Gordon E., Jr. TI Properties of impurity-bearing ferrihydrite II: Insights into the surface structure and composition of pure, Al- and Si-bearing ferrihydrite from Zn(II) sorption experiments and Zn K-edge X-ray absorption spectroscopy SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article ID FINE-STRUCTURE SPECTROSCOPY; HYDROUS FERRIC-OXIDE; AQUEOUS ZN(II); PRECIPITATE GEOMETRY; ZINC SORPTION; ADSORPTION; EXAFS; COMPLEXATION; HEMATITE; FE(III) AB Naturally occurring ferrihydrite often contains impurities such as Al and Si, which can impact its chemical reactivity with respect to metal(loid) adsorption and (in) organic or microbially induced reductive dissolution. However, the surface composition of impure ferrihydrites is not well constrained, and this hinders our understanding of the factors controlling the surface reactivity of these nanophases. In this study, we conducted Zn(II) adsorption experiments combined with Zn K-edge X-ray absorption spectroscopy measurements on pure ferrihydrite (Fh) and Al- or Si-bearing ferrihydrites containing 10 and 20 mol% Al or Si (referred to as 10AlFh, 20AlFh and 10SiFh, 20SiFh) to evaluate Zn(II) uptake in relation to Zn(II) speciation at their surfaces. Overall, Zn(II) uptake at the surface of AlFh is similar to that of pure Fh, and based on Zn K-edge EXAFS data, Zn(II) speciation at the surface of Fh and AlFh also appears similar. Binuclear bidentate Zn-IV-Fe-VI complexes (at similar to 3.46 angstrom (C-2[1]) and similar to 3.25 angstrom (C-2[2])) were identified at low Zn(II) surface coverages from Zn K-edge EXAFS fits. With increasing Zn(II) surface coverage, the number of second-neighbor Fe ions decreased, which was interpreted as indicating the formation of Zn-IV polymers at the ferrihydrite surface, and a deviation from Langmuir uptake behavior. Zn(II) uptake at the surface of SiFh samples was more significant than at Fh and AlFh surfaces, and was attributed to the formation of outer-sphere complexes (on average 24% of sorbed Zn). Although similar Zn-Fe/Zn distances were obtained for the Zn-sorbed SiFh samples, the number of Fe second neighbors was lower in comparison with Fh. The decrease in second-neighbor Fe is most pronounced for sample 20SiFh, suggesting that the amount of reactive surface Fe sites diminishes with increasing Si content. Although our EXAFS results shown here do not provide evidence for the existence of Zn-Al or Zn-Si complexes, their presence is not excluded for Zn-sorbed AlFh or SiFh. The results of this study indicate that Zn(II) interaction with Fh is influenced by the type of impurities associated with this nanomineral, particularly in the case of Si-bearing Fh, and this may have implications for our understanding of metal(loid) mobility in natural systems. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Cismasu, A. Cristina; Levard, Clement; Michel, F. Marc; Brown, Gordon E., Jr.] Stanford Univ, Dept Geol & Environm Sci, Stanford, CA 94305 USA. [Brown, Gordon E., Jr.] SLAC Natl Accelerator Lab, Dept Photon Sci, Menlo Pk, CA 94025 USA. [Brown, Gordon E., Jr.] SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94025 USA. RP Cismasu, AC (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM accismasu@lbl.gov FU DOE-BER [DE-SC0006772]; NSF [EF-0830093]; DOE-BER; Corning Inc. Foundation FX This study was supported by DOE-BER Grant DE-SC0006772 (C. C., G. B.), NSF Grant EF-0830093 (Center for Environmental Implications of Nanotechnology) (C. L., G. B.), DOE-BER Science Focus Area funding to SLAC (M. M., G. B.), and the Corning Inc. Foundation (C. C., G. B.). We are grateful for access to the Stanford Synchrotron Radiation Lightsource (SSRL) at SLAC National Accelerator Laboratory, where we collected our XAS data. SSRL is supported by the Director, Office of Science, Office of Basic Energy Sciences of the US Department of Energy. We wish to thank John Bargar and Joe Rogers for technical support on beam line 11-2 at SSRL, and Guangchao Li (Stanford University) for ICP-OES analyses. NR 48 TC 16 Z9 16 U1 8 U2 64 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD OCT 15 PY 2013 VL 119 BP 46 EP 60 DI 10.1016/j.gca.2013.05.040 PG 15 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA 213EC UT WOS:000324036200004 ER PT J AU Druhan, JL Steefel, CI Williams, KH DePaolo, DJ AF Druhan, Jennifer L. Steefel, Carl I. Williams, Kenneth H. DePaolo, Donald J. TI Calcium isotope fractionation in groundwater: Molecular scale processes influencing field scale behavior SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article ID URANIUM BIOREMEDIATION; CA-44/CA-40 FRACTIONATION; SOLUTION STOICHIOMETRY; BACTERIAL UREOLYSIS; SULFATE REDUCTION; MARINE-SEDIMENTS; CA ISOTOPES; PORE FLUID; GROWTH; PRECIPITATION AB It is the purpose of this study to demonstrate that the molecular scale reaction mechanisms describing calcite precipitation and calcium isotope fractionations under highly controlled laboratory conditions also reproduce field scale measurements of delta Ca-44 in groundwater systems. We present data collected from an aquifer during active carbonate mineral precipitation and develop a reactive transport model capturing the observed chemical and isotopic variations. Carbonate mineral precipitation and associated fluid delta Ca-44 data were measured in multiple clogged well bores during organic carbon amended biogenic reduction of a uranium contaminated aquifer in western Colorado, USA. Secondary mineral formation induced by carbonate alkalinity generated during the biostimulation process lead to substantial permeability reduction in multiple electron-donor injection wells at the field site. These conditions resulted in removal of aqueous calcium from a background concentration of 6 mM to <1 mM while delta Ca-44 enrichment ranged from 1 parts per thousand to greater than 2.5 parts per thousand. The relationship between aqueous calcium removal and isotopic enrichment did not conform to Rayleigh model behavior. Explicit treatment of the individual isotopes of calcium within the CrunchFlow reactive transport code demonstrates that the system did not achieve isotopic reequilibration over the time scale of sample collection. Measured fluid delta Ca-44 values are accurately reproduced by a linear rate law when the Ca2+:CO32- activity ratio remains substantially greater than unity. Variation in the measured delta Ca-44 between wells is shown to originate from a difference in carbonate alkalinity generated in each well bore. The influence of fluid Ca2+:CO32- ratio on the precipitation rate and delta Ca-44 is modeled by coupling the CrunchFlow reactive transport code to an ion by ion growth model. This study presents the first coupled ion-by-ion and reactive transport model for isotopic enrichment and demonstrates that reproducing field-scale delta Ca-44 enrichment in groundwater where Ca2+:CO32- approaches unity is only accomplished by utilizing such a coupled modeling approach. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Druhan, Jennifer L.; DePaolo, Donald J.] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. [Steefel, Carl I.; Williams, Kenneth H.; DePaolo, Donald J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Druhan, JL (reprint author), Stanford Univ, 450 Serra Mall,Braun Hall,Bldg 320, Stanford, CA 94305 USA. EM jdruhan@stanford.edu RI Steefel, Carl/B-7758-2010; Williams, Kenneth/O-5181-2014; Druhan, Jennifer/G-2584-2011 OI Williams, Kenneth/0000-0002-3568-1155; FU U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research [DE-AC02-05CH11231]; U.S. Department of Energy, Office of Science, Subsurface Biogeochemical Research through the Integrated Field Research Challenge (IFRC) at Rifle, Colorado FX This research was supported as part of the Subsurface Science Scientific Focus Area at the Lawrence Berkeley National Laboratory funded by the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research under Award No. DE-AC02-05CH11231 and by the U.S. Department of Energy, Office of Science, Subsurface Biogeochemical Research through the Integrated Field Research Challenge (IFRC) at Rifle, Colorado. The authors wish to thank Shaun Brown, Jim Watkins and Laura Nielsen for helpful discussions, as well as Andrew Jacobson, Edward Tipper and three anonymous reviewers for their thoughtful comments on the manuscript. NR 74 TC 15 Z9 15 U1 8 U2 51 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD OCT 15 PY 2013 VL 119 BP 93 EP 116 DI 10.1016/j.gca.2013.05.022 PG 24 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA 213EC UT WOS:000324036200007 ER PT J AU Zhao, LD Dong, HL Kukkadapu, R Agrawal, A Liu, D Zhang, J Edelmann, RE AF Zhao, Linduo Dong, Hailiang Kukkadapu, Ravi Agrawal, Abinash Liu, Deng Zhang, Jing Edelmann, Richard E. TI Biological oxidation of Fe(II) in reduced nontronite coupled with nitrate reduction by Pseudogulbenkiania sp Strain 2002 SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article ID MICROBIAL REDUCTION; CLAY-MINERALS; FERROUS IRON; SPECTROPHOTOMETRIC DETERMINATION; ANAEROBIC BIOOXIDATION; STRUCTURAL FE(III); ANOXIC CONDITIONS; NEUTRAL PH; BACTERIA; WATER AB The importance of microbial nitrate-dependent Fe(II) oxidation to iron biogeochemistry is well recognized. Past research has focused on oxidation of aqueous Fe2+ and structural Fe(II) in oxides, carbonates, and phosphate, but the importance of structural Fe(II) in phyllosilicates in this reaction is only recently studied. However, the effect of clay mineralogy on the rate and the mechanism of the reaction, and subsequent mineralogical end products are still poorly known. The objective of this research was to study the coupled process of microbial oxidation of Fe(II) in clay mineral nontronite (NAu-2), and nitrate reduction by Pseudogulbenkiania species strain 2002, and to determine mineralogical changes associated with this process. Bio-oxidation experiments were conducted using Fe(II) in microbially reduced nontronite as electron donor and nitrate as electron acceptor in bicarbonate-buffered medium under both growth and nongrowth conditions to investigate cell growth on this process. The extents of Fe(II) oxidation and nitrate reduction were measured by wet chemical methods. X-ray diffraction (XRD), scanning and transmission electron microscopy (SEM and TEM), and Fe-57-Mossbauer spectroscopy were used to observe mineralogical changes associated with Fe(III) reduction and Fe(II) oxidation in NAu-2. The bio-oxidation extent under growth and nongrowth conditions reached 67% and 57%, respectively. Over the same time period, nitrate was completely reduced under both conditions to nitrogen gas (N-2), via an intermediate product nitrite. Abiotic oxidation by nitrite partly accelerated Fe(II) oxidation rate under the growth condition. The oxidized Fe(III) largely remained in the nontronite structure, but secondary minerals such as vivianite, ferrihydrite, and magnetite formed depending on specific experimental conditions. The results of this study highlight the importance of iron-bearing clay minerals in the global nitrogen cycle with potential applications in nitrate removal in natural environments. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Zhao, Linduo; Dong, Hailiang; Zhang, Jing] Miami Univ, Dept Geol & Environm Earth Sci, Oxford, OH 45056 USA. [Dong, Hailiang] China Univ Geosci, Geomicrobiol Lab, State Key Lab Geobiol & Environm Geol, Beijing 100083, Peoples R China. [Kukkadapu, Ravi] Pacific NW Natl Lab, EMSL, Richland, WA 99352 USA. [Agrawal, Abinash] Wright State Univ, Dept Earth & Environm Sci, Dayton, OH 45435 USA. [Liu, Deng] China Univ Geosci, State Key Lab Geobiol & Environm Geol, Wuhan 430074, Peoples R China. [Edelmann, Richard E.] Miami Univ, Ctr Adv Microscopy & Imaging, Oxford, OH 45056 USA. RP Dong, HL (reprint author), Miami Univ, Dept Geol & Environm Earth Sci, Oxford, OH 45056 USA. EM dongh@muohio.edu FU National Science Foundation [EAR 1148039]; Department of Energy's Office of Biological and Environmental Research located at Pacific Northwest National Laboratory; NSF [EAR-0722807] FX The work was supported by a grant from National Science Foundation (EAR 1148039). A portion of the research was performed using EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research located at Pacific Northwest National Laboratory. The JEOL 2100 TEM used in this study was supported by NSF grant EAR-0722807. We are grateful to four anonymous reviewers whose comments significantly improved the quality of the manuscript. NR 67 TC 9 Z9 11 U1 7 U2 94 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 EI 1872-9533 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD OCT 15 PY 2013 VL 119 BP 231 EP 247 DI 10.1016/j.gca.2013.05.033 PG 17 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA 213EC UT WOS:000324036200016 ER PT J AU Kim, WC Kim, JY Ko, JH Kim, J Han, KH AF Kim, Won-Chan Kim, Joo-Yeol Ko, Jae-Heung Kim, Jungmook Han, Kyung-Hwan TI Transcription factor MYB46 is an obligate component of the transcriptional regulatory complex for functional expression of secondary wall-associated cellulose synthases in Arabidopsis thaliana SO JOURNAL OF PLANT PHYSIOLOGY LA English DT Article DE Arabidopsis; Cellulose synthase; MYB46; Secondary wall; Transcription factor ID CELL-WALL; DIRECT TARGET; BIOSYNTHESIS; GENES; XYLEM; NAC; PHENOTYPE; PLANTS; MYB83; SND1 AB Cellulose, the most abundant biopolymer on Earth, is a central component in plant cell walls and highly abundant (up to 50%) in the secondary walls. In Arabidopsis thaliana, the cellulose biosynthesis in the secondary walls is catalyzed by three cellulose synthases CESA4, CESA7 and CESA8. The transcription factor MYB46 and its close homolog MYB83 directly regulate the expression of the three secondary wall cellulose synthases (CESAs). However, it is not known whether MYB46 is the necessary regulator for functional expression of the secondary wall CESAs or one of the multiple transcriptional factors involved in the transcriptional regulatory program. To address this question, we used a series of genetic complementation experiments of the cesa knock-out mutants with the CESA coding sequence driven by either native- or mutated promoter of the genes. The mutant promoters have two nucleotide point mutations in the MYB46 binding cis element (M46RE) such that MYB46 cannot bind to the promoter, while the binding of other known secondary wall transcription factors is not affected. The mutant complementation results showed that MYB46 is essential to restore normal phenotype from the cesa mutants. We conclude that MYB46 is an obligate component of the transcriptional regulatory complex toward the commitment of secondary wall cellulose synthesis in Arabidopsis. (C) 2013 Elsevier GmbH. All rights reserved. C1 [Kim, Won-Chan; Kim, Joo-Yeol; Han, Kyung-Hwan] Michigan State Univ, Dept Hort, E Lansing, MI 48824 USA. [Kim, Won-Chan; Kim, Joo-Yeol; Han, Kyung-Hwan] Michigan State Univ, Dept Forestry, E Lansing, MI 48824 USA. [Kim, Won-Chan; Kim, Joo-Yeol; Han, Kyung-Hwan] Michigan State Univ, DOE Great Lakes Bioenergy Res Ctr, E Lansing, MI 48824 USA. [Kim, Jungmook; Han, Kyung-Hwan] Chonnam Natl Univ, Dept Bioenergy Sci & Technol, Kwangju 500757, South Korea. [Ko, Jae-Heung] Kyung Hee Univ, Dept Plant & Environm New Resources, Yongin 446701, Gyeonggi Do, South Korea. [Ko, Jae-Heung] Kyung Hee Univ, Bioenergy Ctr, Yongin, South Korea. RP Han, KH (reprint author), Michigan State Univ, Dept Hort, E Lansing, MI 48824 USA. EM hanky@msu.edu FU DOE Great Lakes Bioenergy Research Center (DOE Office of Science BER) [DR-FC02-07ER64494]; Ministry of Education, Science and Technology of Korea via the World Class University Project at Chonnam National University [R31-2009-000-20025-0]; Basic Science Research Program through the National Research Foundation of Korea (NRF) [2011-0008840]; Korea Forest Service [S111212L18010] FX This work was funded by the DOE Great Lakes Bioenergy Research Center (DOE Office of Science BER DR-FC02-07ER64494), in part by the Ministry of Education, Science and Technology of Korea via the World Class University Project at Chonnam National University (R31-2009-000-20025-0), and in part by Basic Science Research Program through the National Research Foundation of Korea (NRF) (2011-0008840) and a grant from Korea Forest Service (S111212L18010). The authors would like to thank Drs. Kenneth Keegstra and C.P. Joshi for helpful discussion during the manuscript preparation. NR 24 TC 11 Z9 13 U1 2 U2 39 PU ELSEVIER GMBH, URBAN & FISCHER VERLAG PI JENA PA OFFICE JENA, P O BOX 100537, 07705 JENA, GERMANY SN 0176-1617 J9 J PLANT PHYSIOL JI J. Plant Physiol. PD OCT 15 PY 2013 VL 170 IS 15 BP 1374 EP 1378 DI 10.1016/j.jplph.2013.04.012 PG 5 WC Plant Sciences SC Plant Sciences GA 221LQ UT WOS:000324660800011 PM 23726771 ER PT J AU Friedman, Z Ingalls, J Siirola, JD Watson, JP AF Friedman, Zev Ingalls, Jack Siirola, John D. Watson, Jean-Paul TI Block-oriented modeling of superstructure optimization problems SO COMPUTERS & CHEMICAL ENGINEERING LA English DT Article DE Superstructure optimization; Generalized disjunctive programming; Stochastic programming; Algebraic modeling language ID LANGUAGE AB We present a novel software framework for modeling large-scale engineered systems as mathematical optimization problems. A key motivating feature in such systems is their hierarchical, highly structured topology. Existing mathematical optimization modeling environments do not facilitate the natural expression and manipulation of hierarchically structured systems. Rather, the modeler is forced to "flatten" the system description, hiding structure that may be exploited by solvers, and obfuscating the system that the modeling environment is attempting to represent. To correct this deficiency, we propose a Python-based "block-oriented" modeling approach for representing the discrete components within the system. Our approach is an extension of the Pyomo library for specifying mathematical optimization problems. Through the use of a modeling components library, the block-oriented approach facilitates a clean separation of system superstructure from the details of individual components. This approach also naturally lends itself to expressing design and operational decisions as disjunctive expressions over the component blocks. By expressing a mathematical optimization problem in a block-oriented manner, inherent structure (e.g., multiple scenarios) is preserved for potential exploitation by solvers. In particular, we show that block-structured mathematical optimization problems can be straightforwardly manipulated by decomposition-based multi-scenario algorithmic strategies, specifically in the context of the PySP stochastic programming library. We illustrate our block-oriented modeling approach using a case study drawn from the electricity grid operations domain: unit commitment with transmission switching and N - 1 reliability constraints. Finally, we demonstrate that the overhead associated with block-oriented modeling only minimally increases model instantiation times, and need not adversely impact solver behavior. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Friedman, Zev; Ingalls, Jack; Siirola, John D.; Watson, Jean-Paul] Sandia Natl Labs, Discrete Math & Complex Syst Dept, Albuquerque, NM 87185 USA. RP Siirola, JD (reprint author), Sandia Natl Labs, Discrete Math & Complex Syst Dept, POB 5800,MS 1326, Albuquerque, NM 87185 USA. EM jdsiiro@sandia.gov; jwatson@sandia.gov FU Sandia National Laboratories' Laboratory-Directed Research and Development Program; U.S. Department of Energy's Office of Science; U.S. Department of Energy's Advanced Research Projects Agency-Energy [DE-AR0000214]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia National Laboratories' Laboratory-Directed Research and Development Program, the U.S. Department of Energy's Office of Science (Advanced Scientific Computing Research program), and the U.S. Department of Energy's Advanced Research Projects Agency-Energy (Grant No. DE-AR0000214) funded portions of this work. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. This paper is released as Sandia technical report SAND 2012-8342J. NR 23 TC 4 Z9 4 U1 1 U2 12 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0098-1354 J9 COMPUT CHEM ENG JI Comput. Chem. Eng. PD OCT 15 PY 2013 VL 57 BP 10 EP 23 DI 10.1016/j.compchemeng.2013.04.008 PG 14 WC Computer Science, Interdisciplinary Applications; Engineering, Chemical SC Computer Science; Engineering GA 213CC UT WOS:000324030200003 ER PT J AU Kumar, M Sigdel, AK Gennett, T Berry, JJ Perkins, JD Ginley, DS Packard, CE AF Kumar, Mukesh Sigdel, A. K. Gennett, T. Berry, J. J. Perkins, J. D. Ginley, D. S. Packard, C. E. TI Optimizing amorphous indium zinc oxide film growth for low residual stress and high electrical conductivity SO APPLIED SURFACE SCIENCE LA English DT Article DE Transparent conducting oxide; Amorphous indium zinc oxide; Design of experiment; Residual stress; Flexible TCO's ID THIN-FILMS; ROOM-TEMPERATURE; TRANSPARENT CONDUCTORS; SEMICONDUCTORS; SUBSTRATE; TRANSISTORS; RESISTANCE AB With recent advances in flexible electronics, there is a growing need for transparent conductors with optimum conductivity tailored to the application and nearly zero residual stress to ensure mechanical reliability. Within amorphous transparent conducting oxide (TCO) systems, a variety of sputter growth parameters have been shown to separately impact film stress and optoelectronic properties due to the complex nature of the deposition process. We apply a statistical design of experiments (DOE) approach to identify growth parameter-material property relationships in amorphous indium zinc oxide (a-IZO) thin films and observed large, compressive residual stresses in films grown under conditions typically used for the deposition of highly conductive samples. Power, growth pressure, oxygen partial pressure, and RF power ratio (RF/(RF + DC)) were varied according to a full-factorial test matrix and each film was characterized. The resulting regression model and analysis of variance (ANOVA) revealed significant contributions to the residual stress from individual growth parameters as well as interactions of different growth parameters, but no conditions were found within the initial growth space that simultaneously produced low residual stress and high electrical conductivity. Extrapolation of the model results to lower oxygen partial pressures, combined with prior knowledge of conductivity-growth parameter relationships in the IZO system, allowed the selection of two promising growth conditions that were both empirically verified to achieve nearly zero residual stress and electrical conductivities >1480 S/cm. This work shows that a-IZO can be simultaneously optimized for high conductivity and low residual stress. (C) 2013 Elsevier B.V. All rights reserved. C1 [Kumar, Mukesh; Packard, C. E.] Colorado Sch Mines, Dept Met & Mat Engn, Golden, CO 80401 USA. [Sigdel, A. K.] Univ Denver, Dept Phys & Astron, Denver, CO 80208 USA. [Sigdel, A. K.; Gennett, T.; Berry, J. J.; Perkins, J. D.; Ginley, D. S.; Packard, C. E.] Natl Renewal Energy Lab, Natl Ctr Photovolta, Golden, CO 80401 USA. RP Packard, CE (reprint author), Colorado Sch Mines, Dept Met & Mat Engn, Golden, CO 80401 USA. EM cpackard@mines.edu RI Packard, Corinne/A-9606-2010 OI Packard, Corinne/0000-0002-5815-8586 FU Center for Revolutionary Solar Photoconversion (CRSP); US Department of Energy [DOE-AC36-08GO28308]; National Renewable Energy Laboratory FX We gratefully acknowledge funding from Center for Revolutionary Solar Photoconversion (CRSP) and US Department of Energy under Contract No. DOE-AC36-08GO28308 with the National Renewable Energy Laboratory. NR 39 TC 7 Z9 7 U1 2 U2 92 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0169-4332 J9 APPL SURF SCI JI Appl. Surf. Sci. PD OCT 15 PY 2013 VL 283 BP 65 EP 73 DI 10.1016/j.apsusc.2013.06.019 PG 9 WC Chemistry, Physical; Materials Science, Coatings & Films; Physics, Applied; Physics, Condensed Matter SC Chemistry; Materials Science; Physics GA 207LR UT WOS:000323601700011 ER PT J AU Mao, BH Liua, CH Gao, X Chang, R Liu, Z Wang, SD AF Mao, Bao-Hua Liua, Chang-Hai Gao, Xu Chang, Rui Liu, Zhi Wang, Sui-Dong TI In situ characterization of catalytic activity of graphene stabilized small-sized Pd nanoparticles for CO oxidation SO APPLIED SURFACE SCIENCE LA English DT Article DE Pd nanoparticles; Graphene; Ambient pressure X-ray photoelectron spectroscopy ID HYBRIDS AB The room-temperature ionic liquid assisted sputtering method is utilized to achieve the Pd-nanoparticle (NP)-graphene hybrid. The supported Pd NPs possess uniformly small sizes of 1-2 nm, which create huge surface area with ultralow Pd consumption and high NP stability. The Pd-NP-graphene hybrid is in situ characterized by the ambient pressure X-ray photoelectron spectroscopy using synchrotron radiation, and the results demonstrate high catalytic activity of the hybrid for CO oxidation. The catalytic behavior is reproducible for several catalytic cycles. The present simple and clean approach is promising to produce metal-NP-based high-efficiency catalysts for CO oxidation. (c) 2013 Elsevier B.V. All rights reserved. C1 [Mao, Bao-Hua; Liua, Chang-Hai; Gao, Xu; Wang, Sui-Dong] Soochow Univ, Western Univ Joint Ctr Synchrotron Radiat Res, Inst Funct Nano & Soft Mat FUNSOM, Suzhou 215123, Jiangsu, Peoples R China. [Mao, Bao-Hua; Liua, Chang-Hai; Gao, Xu; Wang, Sui-Dong] Soochow Univ, Inst Funct Nano & Soft Mat FUNSOM, Jiangsu Key Lab Carbon Based Funct Mat & Devices, Suzhou 215123, Jiangsu, Peoples R China. [Mao, Bao-Hua; Chang, Rui; Liu, Zhi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Chang, Rui] Chinese Acad Sci, Shanghai Inst Microsyst & Informat Technol, Shanghai 200050, Peoples R China. RP Liu, Z (reprint author), Soochow Univ, Western Univ Joint Ctr Synchrotron Radiat Res, Inst Funct Nano & Soft Mat FUNSOM, Suzhou 215123, Jiangsu, Peoples R China. EM zliu2@lbl.gov; wangsd@suda.edu.cn RI 刘, 长海/F-9445-2013; Liu, Changhai/B-1577-2015; Wang, Sui-Dong/E-6063-2013; Liu, Zhi/B-3642-2009; GAO, Xu/C-9970-2016; Gao, Xu/S-8258-2016 OI 刘, 长海/0000-0001-6774-5216; Liu, Zhi/0000-0002-8973-6561; GAO, Xu/0000-0002-7491-0758; Gao, Xu/0000-0002-0356-048X FU National Basic Research Development Program of China (973 Program) [2010CB934503, 2011CB808404]; National Natural Science Foundation of China [61006015, 51033007, 61274019]; Natural Science Foundation of Jiangsu Province [BK2010220]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the National Basic Research Development Program of China (973 Program, Nos. 2010CB934503 and 2011CB808404), the National Natural Science Foundation of China (Nos. 61006015, 51033007, and 61274019), and the Natural Science Foundation of Jiangsu Province (No. BK2010220). The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy (No. DE-AC02-05CH11231). NR 23 TC 8 Z9 8 U1 3 U2 100 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0169-4332 J9 APPL SURF SCI JI Appl. Surf. Sci. PD OCT 15 PY 2013 VL 283 BP 1076 EP 1079 DI 10.1016/j.apsusc.2013.07.078 PG 4 WC Chemistry, Physical; Materials Science, Coatings & Films; Physics, Applied; Physics, Condensed Matter SC Chemistry; Materials Science; Physics GA 207LR UT WOS:000323601700154 ER PT J AU Jia, WL Fu, JY Cao, ZY Wang, L Chi, XB Gao, WG Wange, LW AF Jia, Weile Fu, Jiyun Cao, Zongyan Wang, Long Chi, Xuebin Gao, Weiguo Wange, Lin-Wang TI Fast plane wave density functional theory molecular dynamics calculations on multi-GPU machines SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Molecular dynamics; Electronic structure; First-principles; Density functional theory; Plane wave pseudopotential; GPU AB Plane wave pseudopotential (PWP) density functional theory (DFT) calculation is the most widely used method for material simulations, but its absolute speed stagnated due to the inability to use large scale CPU based computers. By a drastic redesign of the algorithm, and moving all the major computation parts into GPU, we have reached a speed of 12 s per molecular dynamics (MD) step for a 512 atom system using 256 GPU cards. This is about 20 times faster than the CPU version of the code regardless of the number of CPU cores used. Our tests and analysis on different GPU platforms and configurations shed lights on the optimal GPU deployments for PWP-DFT calculations. An 1800 step MD simulation is used to study the liquid phase properties of GaInP. (C) 2013 Elsevier Inc. All rights reserved. C1 [Jia, Weile; Fu, Jiyun; Cao, Zongyan; Wang, Long; Chi, Xuebin] Chinese Acad Sci, Comp Network Informat Ctr, Supercomp Ctr, Beijing 100190, Peoples R China. [Jia, Weile; Fu, Jiyun] Univ Chinese Acad Sci, Beijing, Peoples R China. [Gao, Weiguo] Fudan Univ, Sch Math Sci, Shanghai 200433, Peoples R China. [Gao, Weiguo] Fudan Univ, MOE Key Lab Computat Phys Sci, Shanghai 200433, Peoples R China. [Wange, Lin-Wang] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Sci Mat, Berkeley, CA 94720 USA. RP Wange, LW (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Sci Mat, 1 Cyclotron Rd Mail Stop 50F Berkeley, Berkeley, CA 94720 USA. EM jiawl@sccas.cn; fujy@sccas.cn; zycao@sccas.cn; wangl@sccas.cn; chi@sccas.cn; wggao@fudan.edu.cn; lwwang@lbl.gov FU National Basic Research Program of China [2010CB832702]; NSF of China [10972215, 60873113, 11071047]; 863 Program [2010AA012301, 2010AA012402]; CNIC program [CNIC_ZR_201202]; Science and Technology Commission of Shanghai Municipality [09ZR1401900]; Office of Science, Office of Basic Energy Sciences, Materials Science and Engineering Division, of the U.S. Department of Energy (DOE) [DE-AC02-05CH11231]; Office of Science of the Department of Energy [DE-AC05-00OR22725] FX We did like to thank Dr. Zhengji Zhao for helping us to compile the codes on the Titan machine. The numerical calculations are performed on Mole-8.5 and Titan. The work of the first five authors is supported by National Basic Research Program of China 2010CB832702, NSF of China 10972215, 60873113; 863 Program 2010AA012301 and 2010AA012402; CNIC program CNIC_ZR_201202. The work of W. Gao is supported by NSF of China 11071047 and Science and Technology Commission of Shanghai Municipality 09ZR1401900. The work of L. W. Wang is supported by the Director, Office of Science, Office of Basic Energy Sciences, Materials Science and Engineering Division, of the U.S. Department of Energy (DOE) under Contract No. DE-AC02-05CH11231. This research used resources of the Oak Ridge Leadership Computing Facility, located in the National Center for Computational Sciences at Oak Ridge National Laboratory, which is supported by the Office of Science of the Department of Energy under Contract DE-AC05-00OR22725. The computer time on Titan was allocated by the Department of Energy's Innovative and Novel Computational Impact on Theory and Experiment (INCITE) program. NR 25 TC 5 Z9 6 U1 1 U2 26 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 J9 J COMPUT PHYS JI J. Comput. Phys. PD OCT 15 PY 2013 VL 251 BP 102 EP 115 DI 10.1016/j.jcp.2013.05.005 PG 14 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA 194KU UT WOS:000322633000005 ER PT J AU Cleveland, MA Brunner, TA Gentile, NA Keasler, JA AF Cleveland, Mathew A. Brunner, Thomas A. Gentile, Nicholas A. Keasler, Jeffrey A. TI Obtaining identical results with double precision global accuracy on different numbers of processors in parallel particle Monte Carlo simulations SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Numerical Reproducibility; Software extended precision; Parallel; Monte Carlo ID ROBUST AB We describe and compare different approaches for achieving numerical reproducibility in photon Monte Carlo simulations. Reproducibility is desirable for code verification, testing, and debugging. Parallelism creates a unique problem for achieving reproducibility in Monte Carlo simulations because it changes the order in which values are summed. This is a numerical problem because double precision arithmetic is not associative. Parallel Monte Carlo, both domain replicated and decomposed simulations, will run their particles in a different order during different runs of the same simulation because the non-reproducibility of communication between processors. In addition, runs of the same simulation using different domain decompositions will also result in particles being simulated in a different order. In [1], a way of eliminating non-associative accumulations using integer tallies was described. This approach successfully achieves reproducibility at the cost of lost accuracy by rounding double precision numbers to fewer significant digits. This integer approach, and other extended and reduced precision reproducibility techniques, are described and compared in this work. Increased precision alone is not enough to ensure reproducibility of photon Monte Carlo simulations. Non-arbitrary precision approaches require a varying degree of rounding to achieve reproducibility. For the problems investigated in this work double precision global accuracy was achievable by using 100 bits of precision or greater on all unordered sums which where subsequently rounded to double precision at the end of every time-step. (C) 2013 Elsevier Inc. All rights reserved. C1 [Cleveland, Mathew A.; Brunner, Thomas A.; Gentile, Nicholas A.; Keasler, Jeffrey A.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Cleveland, MA (reprint author), Lawrence Livermore Natl Lab, L-405,POB 808, Livermore, CA 94550 USA. EM cleveland7@llnl.gov FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 16 TC 2 Z9 2 U1 1 U2 4 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 J9 J COMPUT PHYS JI J. Comput. Phys. PD OCT 15 PY 2013 VL 251 BP 223 EP 236 DI 10.1016/j.jcp.2013.05.041 PG 14 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA 194KU UT WOS:000322633000011 ER PT J AU Gao, MC Ouyang, LZ Dogan, ON AF Gao, Michael C. Ouyang, Lizhi Dogan, Oemer N. TI First principles screening of B2 stabilizers in CuPd-based hydrogen separation membranes: (1) Substitution for Pd SO JOURNAL OF ALLOYS AND COMPOUNDS LA English DT Article DE First-principles calculations; B2 CuPd; Hydrogen separation membranes; Hume-Rothery rules; Charge transfer; Electronegativity ID DENSITY-FUNCTIONAL THEORY; 1ST-PRINCIPLES CALCULATIONS; ALLOY MEMBRANES; PURIFICATION MEMBRANES; PD(111) SURFACE; TERNARY ALLOYS; METALS; SYSTEM; DECOMPOSITION; TEMPERATURES AB We report here a screening study using first-principles method in an attempt to identify ternary elements that can extend the CuPd B2 phase field at reduced Pd contents and thus lower cost. A total of 37 alloying elements are included for unbiased screening. The results show that addition of Mg, Al, Sc, Ti, Y, Hf, Zr, Ga, La, and Zn lowers the enthalpy of formation of the B2 phase noticeably. The atomic size, electronic density of states, charge transfer, and electronegativity are analyzed to interpret the results. Compromise between enthalpy and solubility suggests additional potential alloying elements: V, Fe, Cr, Nb, Ta, and Mn. To assess the effects of alloying on mechanical properties, we calculated the equation of states and elastic constants of 10 example alloys at 6.25 at% solute contents. (C) 2013 Elsevier B.V. All rights reserved. C1 [Gao, Michael C.; Dogan, Oemer N.] Natl Energy Technol Lab, Albany, OR 97321 USA. [Gao, Michael C.] URS Corp, Albany, OR 97321 USA. [Ouyang, Lizhi] Tennessee State Univ, Dept Phys & Math, Nashville, TN 37209 USA. RP Gao, MC (reprint author), Natl Energy Technol Lab, 1450 Queen Ave SW, Albany, OR 97321 USA. EM michael.gao@contr.netl.doe.gov FU Fuels Program as well as the Innovative Processing and Technologies Program of Strategic Center for Coal at DOE National Energy Technology Laboratory [DE-FE0004000]; Pittsburgh Supercomputing Center (PSC) [DMR110001P]; Texas Advanced Computing Center (TACC) [DMR120048]; Extreme Science and Engineering Discovery Environment (XSEDE); National Science Foundation [OCI-1053575] FX This technical effort was performed in support of the Fuels Program as well as the Innovative Processing and Technologies Program of Strategic Center for Coal at DOE National Energy Technology Laboratory under the RES contract DE-FE0004000. MCG thanks Drs. David Alman and De Nyago Tafen at NETL for carefully reviewing this manuscript and Prof. Michael Widom at Carnegie Mellon University and Dr. Bryan Morealle at NETL for useful discussions. This work used the computing facility at Pittsburgh Supercomputing Center (PSC) through Award DMR110001P and Texas Advanced Computing Center (TACC) through Award# DMR120048 by the Extreme Science and Engineering Discovery Environment (XSEDE), which is supported by National Science Foundation Grant Number OCI-1053575. NR 53 TC 3 Z9 3 U1 0 U2 20 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0925-8388 J9 J ALLOY COMPD JI J. Alloy. Compd. PD OCT 15 PY 2013 VL 574 BP 368 EP 376 DI 10.1016/j.jallcom.2013.05.126 PG 9 WC Chemistry, Physical; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Chemistry; Materials Science; Metallurgy & Metallurgical Engineering GA 182NG UT WOS:000321749600061 ER PT J AU Guo, M Kim, GH White, RE AF Guo, Meng Kim, Gi-Heon White, Ralph E. TI A three-dimensional multi-physics model for a Li-ion battery SO JOURNAL OF POWER SOURCES LA English DT Article DE Li-ion; Battery module; 3D model; Pseudo-2D ID SOLID-PHASE DIFFUSION; THERMAL-MODEL; CELL; PERFORMANCE; REFORMULATION; BEHAVIOR AB A multi-geometry and multi-physics model is developed for a Li-ion battery module which includes three cells connected in series by electrical busbars. The model can be used to predict the 3D profiles of the electrical potentials and temperature in the battery. The physics-based porous electrode (P2D) model is used to predict the electrochemical behavior of the cells, and the coupling between the P2D model and the electrical/thermal equations is simplified through a linear approximation method. This approximation is useful at rates of at least 5 C and reduces the computation time significantly. The anisotropic conductive properties for the regions where conductors are separately arrayed are discussed in detail, and the model predictions are presented and discussed. (C) 2013 Elsevier B.V. All rights reserved. C1 [Guo, Meng; White, Ralph E.] Univ S Carolina, Dept Chem Engn, Columbia, SC 29208 USA. [Kim, Gi-Heon] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP White, RE (reprint author), 301 Main St, Columbia, SC 29208 USA. EM white@cec.sc.edu RI Guo, Meng/L-8432-2014 NR 21 TC 20 Z9 21 U1 5 U2 74 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD OCT 15 PY 2013 VL 240 BP 80 EP 94 DI 10.1016/j.jpowsour.2013.03.170 PG 15 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA 183GY UT WOS:000321803700012 ER PT J AU Lee, ES Huq, A Manthiram, A AF Lee, Eun-Sung Huq, Ashfia Manthiram, Arumugam TI Understanding the effect of synthesis temperature on the structural and electrochemical characteristics of layered-spinel composite cathodes for lithium-ion batteries SO JOURNAL OF POWER SOURCES LA English DT Article DE Lithium-ion batteries; Layered-spinel composite cathodes; Structural analysis; Cation ordering ID NICKEL MANGANESE OXIDES; HIGH-VOLTAGE; CRYSTAL-STRUCTURE; ELECTRODE MATERIALS; NI; LIMN1.5NI0.5O4; LI2MNO3; CHARGE; CO; LINI0.5MN1.5O4-DELTA AB The effect of synthesis temperature on the structural and electrochemical characteristics of the layered-spinel composite cathode system xLi[Li0.2Mn0.6Ni02]O-2-(1 - x)Li[Mn1.5Ni0.5]O-4 (0 <= x <= 1) has been investigated. With a joint neutron diffraction (ND) and X-ray diffraction (XRD) Rietveld refinement method, the composition and weight percent variations of the layered and spinel phases in this composite cathode system have been obtained as a function of x and synthesis temperature. While no significant composition and weight percent variations are found with the synthesis temperature, the electrochemical characteristics of both the layered and spinel phases in the composites are significantly affected by the synthesis temperature. In contrast to the layered sample (x = 1), the capacity of the layered phase in the composites increases with decreasing synthesis temperature due to an increase in surface area. Conversely, the effect of synthesis temperature on the spinel phase is similar in both the spinel sample (x = 0) and the composite samples. However, the lower synthesis temperature increases the cation ordering in the 16d octahedral sites of the spinet phase, which changes the voltage profiles below 3 V due to the decrease in the lattice distortion during lithium ion insertion into the empty 16c octahedral sites. (C) 2013 Elsevier B.V. All rights reserved. C1 [Lee, Eun-Sung; Manthiram, Arumugam] Univ Texas Austin, Mat Sci & Engn Program, Austin, TX 78712 USA. [Lee, Eun-Sung; Manthiram, Arumugam] Univ Texas Austin, Texas Mat Inst, Austin, TX 78712 USA. [Huq, Ashfia] Oak Ridge Natl Lab, Chem & Engn Mat Div, Neutron Sci Directorate, Oak Ridge, TN 37831 USA. RP Manthiram, A (reprint author), Univ Texas Austin, Mat Sci & Engn Program, Austin, TX 78712 USA. EM rmanth@mail.utexas.edu RI Huq, Ashfia/J-8772-2013 OI Huq, Ashfia/0000-0002-8445-9649 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-SC0005397]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX This work was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under award number DE-SC0005397. Neutron diffraction portion of this research at ORNL's Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. NR 47 TC 26 Z9 27 U1 3 U2 233 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD OCT 15 PY 2013 VL 240 BP 193 EP 203 DI 10.1016/j.jpowsour.2013.04.010 PG 11 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA 183GY UT WOS:000321803700025 ER PT J AU Liu, HD Fell, CR An, K Cai, L Meng, YS AF Liu, Haodong Fell, Christopher R. An, Ke Cai, Lu Meng, Ying Shirley TI In-situ neutron diffraction study of the xLi(2)MnO(3)center dot(1-x)LiMO2 (x=0, 0.5; M = Ni, Mn, Co) layered oxide compounds during electrochemical cycling SO JOURNAL OF POWER SOURCES LA English DT Article DE Lithium-ion battery; In-situ neutron diffraction; Layered oxide cathode; Graphite anode ID LITHIUM-ION BATTERIES; NICKEL MANGANESE OXIDES; X-RAY-DIFFRACTION; ELECTRODE MATERIALS; INSERTION MATERIAL; STRUCTURAL-CHANGES; LICO1/3NI1/3MN1/3O2; INTERCALATION; CATHODE; LI2MNO3 AB The layered oxide compounds xLi(2)MnO(3)center dot(1 - x)LiMO2 (M = Ni, Mn, Co) are of great interest as positive electrode materials for high energy density lithium-ion batteries. In-situ neutron diffraction was carried out to compare the structural changes between the classical layered compound Li[Ni1/3Mn1/3Co1/3]O-2 (x = 0) and lithium-excess layered compound Li[Li0.2Ni0.18Mn0.53Co0.1]O-2 (x = 0.5) during electrochemical cycling. In this work, lab made pouch cells were built for the in-situ study and graphite was used as the anode material. Irreversible structural change of Li[Li0.2Ni0.18Mn0.53Co0.1]O-2 during first charge (4.7 V)/discharge cycle (2.0 V) was indicated by dynamic changes in lattice d-spacing, while the Li[Ni1/3Mn1/3Co1/3]O-2 showed completely reversible structural evolution between 4.4 V and 2.5 V. Ex-situ neutron powder diffraction was performed on both pristine and chemically delithiated lithium-excess layered compounds to better understand the irreversible structure change. (C) 2013 Published by Elsevier B.V. C1 [Liu, Haodong; Meng, Ying Shirley] Univ Calif San Diego, Dept NanoEngn, La Jolla, CA 92121 USA. [Fell, Christopher R.] Johnson Controls Inc, Global Technol & Innovat, Power Solut, Milwaukee, WI 53209 USA. [An, Ke; Cai, Lu] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37830 USA. RP Meng, YS (reprint author), Univ Calif San Diego, Dept NanoEngn, La Jolla, CA 92121 USA. EM shirleymeng@ucsd.edu RI An, Ke/G-5226-2011 OI An, Ke/0000-0002-6093-429X FU office of Basic Energy Sciences (BES); China Scholarship Council [2011631005]; Office of Vehicle Technologies of the U.S. DOE [DE-AC02-05CH11231]; Batteries for Advanced Transportation Technologies (BATT) Program [7056412]; Division of Materials Science, the office of BES, Office of Science of DOE; Office of Science of the U.S. Department of Energy (DOE) FX The neutron experiments benefit from the SNS and HFIR user facilities sponsored by the office of Basic Energy Sciences (BES), the Office of Science of the U.S. Department of Energy (DOE). H. Liu acknowledges the financial support from China Scholarship Council under Award Number 2011631005. UCSD's efforts are supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. DOE under Contract No. DE-AC02-05CH11231, Subcontract No. 7056412 under the Batteries for Advanced Transportation Technologies (BATT) Program. L. Cai acknowledges the financial support from the Division of Materials Science, the office of BES, Office of Science of DOE. NR 32 TC 33 Z9 33 U1 4 U2 154 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD OCT 15 PY 2013 VL 240 BP 772 EP 778 DI 10.1016/j.jpowsour.2013.04.149 PG 7 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA 183GY UT WOS:000321803700095 ER PT J AU Agnese, R Anderson, AJ Balakishiyeva, D Thakur, RB Bauer, DA Borgland, A Brandt, D Brink, PL Bunker, R Cabrera, B Caldwell, DO Cerdeno, DG Chagani, H Cherry, M Cooley, J Cornell, B Crewdson, CH Cushman, P Daal, M Di Stefano, PCF Silva, EDE Doughty, T Esteban, L Fallows, S Figueroa-Feliciano, E Fox, J Fritts, M Godfrey, GL Golwala, SR Hall, J Harris, HR Hasi, J Hertel, SA Hines, BA Hofer, T Holmgren, D Hsu, L Huber, ME Jastram, A Kamaev, O Kara, B Kelsey, MH Kenany, SA Kennedy, A Kenney, CJ Kiveni, M Koch, K Loer, B Asamar, EL Mahapatra, R Mandic, V Martinez, C McCarthy, KA Mirabolfathi, N Moffatt, RA Moore, DC Nadeau, P Nelson, RH Novak, L Page, K Partridge, R Pepin, M Phipps, A Prasad, K Pyle, M Qiu, H Radpour, R Rau, W Redl, P Reisetter, A Resch, RW Ricci, Y Saab, T Sadoulet, B Sander, J Schmitt, R Schneck, K Schnee, RW Scorza, S Seitz, D Serfass, B Shank, B Speller, D Tomada, A Villano, AN Welliver, B Wright, DH Yellin, S Yen, JJ Young, BA Zhang, J AF Agnese, R. Anderson, A. J. Balakishiyeva, D. Thakur, R. Basu Bauer, D. A. Borgland, A. Brandt, D. Brink, P. L. Bunker, R. Cabrera, B. Caldwell, D. O. Cerdeno, D. G. Chagani, H. Cherry, M. Cooley, J. Cornell, B. Crewdson, C. H. Cushman, P. Daal, M. Di Stefano, P. C. F. Do Couto E Silva, E. Doughty, T. Esteban, L. Fallows, S. Figueroa-Feliciano, E. Fox, J. Fritts, M. Godfrey, G. L. Golwala, S. R. Hall, J. Harris, H. R. Hasi, J. Hertel, S. A. Hines, B. A. Hofer, T. Holmgren, D. Hsu, L. Huber, M. E. Jastram, A. Kamaev, O. Kara, B. Kelsey, M. H. Kenany, S. A. Kennedy, A. Kenney, C. J. Kiveni, M. Koch, K. Loer, B. Lopez Asamar, E. Mahapatra, R. Mandic, V. Martinez, C. McCarthy, K. A. Mirabolfathi, N. Moffatt, R. A. Moore, D. C. Nadeau, P. Nelson, R. H. Novak, L. Page, K. Partridge, R. Pepin, M. Phipps, A. Prasad, K. Pyle, M. Qiu, H. Radpour, R. Rau, W. Redl, P. Reisetter, A. Resch, R. W. Ricci, Y. Saab, T. Sadoulet, B. Sander, J. Schmitt, R. Schneck, K. Schnee, R. W. Scorza, S. Seitz, D. Serfass, B. Shank, B. Speller, D. Tomada, A. Villano, A. N. Welliver, B. Wright, D. H. Yellin, S. Yen, J. J. Young, B. A. Zhang, J. CA SuperCDMS Collaboration TI Demonstration of surface electron rejection with interleaved germanium detectors for dark matter searches SO APPLIED PHYSICS LETTERS LA English DT Article ID 730 KG DAYS; DISCRIMINATION AB The SuperCDMS experiment in the Soudan Underground Laboratory searches for dark matter with a 9-kg array of cryogenic germanium detectors. Symmetric sensors on opposite sides measure both charge and phonons from each particle interaction, providing excellent discrimination between electron and nuclear recoils, and between surface and interior events. Surface event rejection capabilities were tested with two Pb-210 sources producing similar to 130 beta decays/hr. In similar to 800 live hours, no events leaked into the 8-115 keV signal region, giving upper limit leakage fraction 1.7 x 10(-5) at 90% C.L., corresponding to <0.6 surface event background in the future 200-kg SuperCDMS SNOLAB experiment. (C) 2013 AIP Publishing LLC. C1 [Agnese, R.; Balakishiyeva, D.; Saab, T.; Welliver, B.] Univ Florida, Dept Phys, Gainesville, FL 32611 USA. [Anderson, A. J.; Figueroa-Feliciano, E.; Hertel, S. A.; McCarthy, K. A.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Thakur, R. Basu; Bauer, D. A.; Holmgren, D.; Hsu, L.; Loer, B.; Schmitt, R.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Thakur, R. Basu] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Borgland, A.; Brandt, D.; Brink, P. L.; Do Couto E Silva, E.; Godfrey, G. L.; Hasi, J.; Kelsey, M. H.; Kenney, C. J.; Partridge, R.; Resch, R. W.; Schneck, K.; Tomada, A.; Wright, D. H.] SLAC Natl Accelerator Lab, Kavli Inst Particle Astrophys & Cosmol, Menlo Pk, CA 94025 USA. [Bunker, R.; Kiveni, M.; Schnee, R. W.] Syracuse Univ, Dept Phys, Syracuse, NY 13244 USA. [Cabrera, B.; Cherry, M.; Moffatt, R. A.; Novak, L.; Redl, P.; Shank, B.; Yellin, S.; Yen, J. J.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Caldwell, D. O.] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA. [Cerdeno, D. G.; Esteban, L.; Lopez Asamar, E.] Univ Autonoma Madrid, Dept Fis Teor, E-28049 Madrid, Spain. [Cerdeno, D. G.; Esteban, L.; Lopez Asamar, E.] Univ Autonoma Madrid, Inst Fis Teor UAM CSIC, E-28049 Madrid, Spain. [Chagani, H.; Cushman, P.; Fallows, S.; Fritts, M.; Hofer, T.; Kennedy, A.; Koch, K.; Mandic, V.; Pepin, M.; Radpour, R.; Villano, A. N.; Zhang, J.] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Cooley, J.; Kara, B.; Qiu, H.; Scorza, S.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Cornell, B.; Golwala, S. R.; Moore, D. C.; Nelson, R. H.] CALTECH, Div Phys Math & Astron, Pasadena, CA 91125 USA. [Crewdson, C. H.; Di Stefano, P. C. F.; Fox, J.; Kamaev, O.; Martinez, C.; Nadeau, P.; Page, K.; Rau, W.; Ricci, Y.] Queens Univ, Dept Phys, Kingston, ON K7L 3N6, Canada. [Daal, M.; Doughty, T.; Kenany, S. A.; Mirabolfathi, N.; Phipps, A.; Pyle, M.; Sadoulet, B.; Seitz, D.; Serfass, B.; Speller, D.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Hall, J.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Harris, H. R.; Jastram, A.; Mahapatra, R.; Prasad, K.; Sander, J.] Texas A&M Univ, Dept Phys, College Stn, TX 77843 USA. [Hines, B. A.; Huber, M. E.] Univ Colorado, Dept Phys, Denver, CO 80217 USA. [Reisetter, A.] Univ Evansville, Dept Phys, Evansville, IN 47722 USA. [Sadoulet, B.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Young, B. A.] Santa Clara Univ, Dept Phys, Santa Clara, CA 95053 USA. RP Agnese, R (reprint author), Univ Florida, Dept Phys, Gainesville, FL 32611 USA. RI Pyle, Matt/E-7348-2015; Hall, Jeter/E-9294-2015; OI Pyle, Matt/0000-0002-3490-6754; Holmgren, Donald/0000-0001-6701-7737; Cerdeno, David G./0000-0002-7649-1956 FU NSF [ECS-0335765]; National Science Foundation [AST-9978911, NSF-0847342, PHY-1102795, NSF-1151869, PHY-0542066, PHY-0503729, PHY-0503629, PHY-0503641, PHY-0504224, PHY-0705052, PHY-0801708, PHY-0801712, PHY-0802575, PHY-0847342, PHY-0855299, PHY-0855525, PHY-1205898]; Department of Energy [DE-AC03-76SF00098, DE-FG02-92ER40701, DE-FG02-94ER40823, DE-FG03-90ER40569, DE-FG03-91ER40618, DE-SC0004022]; NSERC Canada [SAPIN 341314, SAPPJ 386399]; MULTIDARK [CSD2009-00064, FPA2012-34694]; Fermi Research Alliance, LLC [De-AC02-07CH11359]; United States Department of Energy [DE-AC02-76SF00515] FX The SuperCDMS collaboration gratefully acknowledges the technical assistance from Jim Beaty and the staff of the Soudan Underground Laboratory and the Minnesota Department of Natural Resources. These iZIP detectors are fabricated in the Stanford Nanofabrication Facility, which is a member of the National Nanofabrication Infrastructure Network sponsored by NSF under Grant ECS-0335765. This work is supported in part by the National Science Foundation (Grant Nos. AST-9978911, NSF-0847342, PHY-1102795, NSF-1151869, PHY-0542066, PHY-0503729, PHY-0503629, PHY-0503641, PHY-0504224, PHY-0705052, PHY-0801708, PHY-0801712, PHY-0802575, PHY-0847342, PHY-0855299, PHY-0855525, and PHY-1205898), by the Department of Energy (Contract Nos. DE-AC03-76SF00098, DE-FG02-92ER40701, DE-FG02-94ER40823, DE-FG03-90ER40569, DE-FG03-91ER40618, and DE-SC0004022), by NSERC Canada (Grant Nos. SAPIN 341314 and SAPPJ 386399), and by MULTIDARK CSD2009-00064 and FPA2012-34694. Fermilab is operated by Fermi Research Alliance, LLC under Contract No. De-AC02-07CH11359, while SLAC is operated under Contract No. DE-AC02-76SF00515 with the United States Department of Energy. NR 32 TC 17 Z9 17 U1 0 U2 18 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD OCT 14 PY 2013 VL 103 IS 16 AR 164105 DI 10.1063/1.4826093 PG 5 WC Physics, Applied SC Physics GA 241EH UT WOS:000326148700104 ER PT J AU Dyer, GC Nordquist, CD Cich, MJ Ribaudo, T Grine, AD Fuller, CT Reno, JL Wanke, MC AF Dyer, Gregory C. Nordquist, Christopher D. Cich, Michael J. Ribaudo, Troy Grine, Albert D. Fuller, Charles T. Reno, John L. Wanke, Michael C. TI Position and mode dependent coupling of terahertz quantum cascade laser fields to an integrated diode SO APPLIED PHYSICS LETTERS LA English DT Article ID HETERODYNE RECEIVER; SCHOTTKY DIODE AB A Schottky diode integrated into a terahertz quantum cascade laser waveguide couples directly to the internal laser fields. In a multimode laser, the diode response is correlated with both the instantaneous power and the coupling strength to the diode of each lasing mode. Measurements of the rectified response of diodes integrated in two quantum cascade laser cavities at different locations indicate that the relative diode position strongly influences the laser-diode coupling. (C) 2013 AIP Publishing LLC. C1 [Dyer, Gregory C.; Nordquist, Christopher D.; Cich, Michael J.; Ribaudo, Troy; Grine, Albert D.; Fuller, Charles T.; Reno, John L.; Wanke, Michael C.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Dyer, GC (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM mcwanke@sandia.gov FU Sandia laboratory directed research and development (LDRD) program; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported by the Sandia laboratory directed research and development (LDRD) program. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 18 TC 1 Z9 1 U1 1 U2 14 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD OCT 14 PY 2013 VL 103 IS 16 AR 161109 DI 10.1063/1.4825214 PG 4 WC Physics, Applied SC Physics GA 241EH UT WOS:000326148700009 ER PT J AU Vilayurganapathy, S Nandasiri, MI Joly, AG El-Khoury, PZ Varga, T Coffey, G Schwenzer, B Pandey, A Kayani, A Hess, WP Thevuthasan, S AF Vilayurganapathy, Subramanian Nandasiri, Manjula I. Joly, Alan G. El-Khoury, Patrick Z. Varga, Tamas Coffey, Greg Schwenzer, Birgit Pandey, Archana Kayani, Asghar Hess, Wayne P. Thevuthasan, Suntharampillai TI Silver nanorod arrays for photocathode applications SO APPLIED PHYSICS LETTERS LA English DT Article ID TRANSMISSION ELECTRON-MICROSCOPY; NANOWIRE ARRAYS; NANOMATERIALS; TEMPLATE; DYNAMICS AB We explore the use of plasmonic Ag nanorod arrays featuring enhanced photoemission as high-brightness photocathode material. Silver nanorod arrays are synthesized by the direct current electrodeposition method and their dimensionality, uniformity, crystallinity, and oxide/impurity content are characterized. The yielded arrays exhibit greatly enhanced two-photon photoemission under 400 nm femtosecond pulsed laser excitation. Plasmonic field enhancement in the array produces photoemission hot spots that are mapped using photoemission electron microscopy. The relative photoemission enhancement of nanorod hot spots relative to that of a flat Ag thin film is found to range between 10(2) and 3 x 10(3). (C) 2013 AIP Publishing LLC. C1 [Vilayurganapathy, Subramanian; Nandasiri, Manjula I.; Varga, Tamas; Pandey, Archana; Thevuthasan, Suntharampillai] Pacific NW Natl Lab, Environm & Mol Sci Lab, Richland, WA 99352 USA. [Vilayurganapathy, Subramanian; Nandasiri, Manjula I.; Kayani, Asghar] Western Michigan Univ, Kalamazoo, MI 49008 USA. [Joly, Alan G.; El-Khoury, Patrick Z.; Schwenzer, Birgit; Hess, Wayne P.] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. [Coffey, Greg] Pacific NW Natl Lab, Energy Proc & Mat Div, Richland, WA 99352 USA. RP Vilayurganapathy, S (reprint author), Pacific NW Natl Lab, Environm & Mol Sci Lab, POB 999, Richland, WA 99352 USA. EM wayne.hess@pnnl.gov RI Vilayur Ganapathy, Subramanian/A-1670-2013; OI Schwenzer, Birgit/0000-0002-7872-1372 FU Department of Energy's Office of Biological and Environmental; Chemical Imaging Initiative FX This research used EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental and located at Pacific Northwest National Laboratory (PNNL) and was supported by the Chemical Imaging Initiative conducted under the Laboratory Directed Research and Development Program. PNNL is a multiprogram national laboratory operated by Battelle Memorial Institute for the U.S. Department of Energy. NR 26 TC 1 Z9 1 U1 4 U2 47 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD OCT 14 PY 2013 VL 103 IS 16 AR 161112 DI 10.1063/1.4825262 PG 5 WC Physics, Applied SC Physics GA 241EH UT WOS:000326148700012 ER PT J AU Drews, AM Cademartiri, L Whitesides, GM Bishop, KJM AF Drews, Aaron M. Cademartiri, Ludovico Whitesides, George M. Bishop, Kyle J. M. TI Electric winds driven by time oscillating corona discharges SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID DIELECTRIC BARRIER DISCHARGE; INDUCED FLOW VELOCITY; ATMOSPHERIC-PRESSURE; PLASMA ACTUATORS; ELECTROSTATIC PRECIPITATORS; ELECTROHYDRODYNAMIC FORCE; NEGATIVE CORONA; GLOW-DISCHARGE; HEAT-TRANSFER; AIR AB We investigate the formation of steady gas flows-so-called electric winds-created by point-plane corona discharges driven by time oscillating (ac) electric fields. By varying the magnitude and frequency of the applied field, we identify two distinct scaling regimes: (i) a low frequency (dc) regime and (ii) a high frequency (ac) regime. These experimental observations are reproduced and explained by a theoretical model describing the transport and recombination of ions surrounding the discharge and their contribution to the measured wind velocity. The two regimes differ in the spatial distribution of ions and in the process by which ions are consumed. Interestingly, we find that ac corona discharges generate strong electric forces localized near the tip of the point electrode, while dc corona discharges generate weaker forces distributed throughout the interelectrode region. Consequently, the velocity of the electric winds (>1 m/s) generated by ac discharges is largely independent of the position of the counter electrode. The unified theoretical description of dc and ac electric winds presented here reconciles previous observations of winds driven by dc corona and ac dielectric barrier discharges; insights from the model should also prove useful in the design of other plasma actuators. (C) 2013 AIP Publishing LLC. C1 [Drews, Aaron M.; Bishop, Kyle J. M.] Penn State Univ, Dept Chem Engn, University Pk, PA 16802 USA. [Cademartiri, Ludovico; Whitesides, George M.] Harvard Univ, Dept Chem & Chem Biol, Cambridge, MA 02138 USA. [Cademartiri, Ludovico] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. [Cademartiri, Ludovico] Iowa State Univ, Dept Chem & Biol Engn, Ames, IA 50011 USA. [Cademartiri, Ludovico] US DOE, Ames Lab, Ames, IA 50011 USA. [Whitesides, George M.] Harvard Univ, Kavli Inst, Cambridge, MA 02138 USA. RP Bishop, KJM (reprint author), Penn State Univ, Dept Chem Engn, University Pk, PA 16802 USA. EM kjmbishop@engr.psu.edu RI Bishop, Kyle/F-1742-2010; Cademartiri, Ludovico/A-4142-2008 OI Cademartiri, Ludovico/0000-0001-8805-9434 FU Defense Advanced Research Projects Agency [W944NF-09-1-0005]; Non-equilibrium Energy Research Center (NERC)-an Energy Frontier Research Center; U.S. Department of Energy [DE-SC0000989]; Iowa State University FX This work was supported by the Defense Advanced Research Projects Agency under Grant No. W944NF-09-1-0005, and by the Non-equilibrium Energy Research Center (NERC)-an Energy Frontier Research Center funded by the U.S. Department of Energy under Award No. DE-SC0000989. L.C. is grateful to Iowa State University for startup funding. NR 42 TC 16 Z9 16 U1 4 U2 51 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD OCT 14 PY 2013 VL 114 IS 14 AR 143302 DI 10.1063/1.4824748 PG 7 WC Physics, Applied SC Physics GA 236FI UT WOS:000325780400008 ER PT J AU Hong, L Li, YL Wu, PP Chen, LQ AF Hong, Liang Li, Yulan Wu, Pingping Chen, Long-Qing TI Minimum tetragonality in PbTiO3/BaTiO3 ferroelectric superlattices SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID EPITAXIAL BATIO3/SRTIO3 SUPERLATTICES; POLARIZATION ENHANCEMENT; THIN-FILMS AB PbTiO3/BaTiO3 ferroelectric superlattices commensurately constrained by a SrTiO3 substrate are studied using both phenomenological theory and phase field simulations. It is found that the spontaneous polarization of the superlattice does not vary significantly with volume fraction until PbTiO3 becomes the majority of the superlattice. A minimum tetragonality exists at room temperature when the PbTiO3 volume fraction is around 90%, resulted from its different sensitivity to epitaxial strains and the electrostatic coupling of the two polarized layers in this PbTiO3/BaTiO3 superlattice. (C) 2013 AIP Publishing LLC. C1 [Hong, Liang; Wu, Pingping; Chen, Long-Qing] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. [Li, Yulan] Pacific NW Natl Lab, Richland, WA 99352 USA. [Wu, Pingping] Univ Sci & Technol Beijing, Dept Phys, Beijing 100083, Peoples R China. RP Hong, L (reprint author), Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. EM lxh42@psu.edu RI Hong, Liang/K-5673-2013; Chen, LongQing/I-7536-2012 OI Chen, LongQing/0000-0003-3359-3781 FU NSF [DMR-0820404, DMR-1210588, DMR-1006541, OCI-0821527]; instrumentation (cyberstar Linux cluster) FX This work was supported by the NSF through grants DMR-0820404, DMR-1210588, and DMR-1006541. The computer simulations were carried out on the LION and cyberstar clusters at the Pennsylvania State University, in part supported by instrumentation (cyberstar Linux cluster) funded by the NSF through Grant OCI-0821527. NR 24 TC 1 Z9 1 U1 1 U2 34 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD OCT 14 PY 2013 VL 114 IS 14 AR 144103 DI 10.1063/1.4824922 PG 4 WC Physics, Applied SC Physics GA 236FI UT WOS:000325780400038 ER PT J AU Lee, WJ Chang, JG Yang, AC Wang, YT Su, WS Wang, CZ Ho, KM AF Lee, Wen-Jay Chang, Jee-Gong Yang, An-Cheng Wang, Yeng-Tseng Su, Wan-Sheng Wang, Cai-Zhuang Ho, Kai-Ming TI Influence of oriented topological defects on the mechanical properties of carbon nanotube heterojunctions SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID INTRAMOLECULAR JUNCTIONS; TEMPERATURE; SIMULATIONS; ALGORITHM; DYNAMICS; DEVICES AB The mechanical properties of finite-length (5,0)/(8,0) single-walled carbon nanotube (SWCNT) heterojunctions with manipulated topological defects are investigated using molecular dynamics simulation calculations. The results show that the mechanical properties and deformation behavior of SWCNT heterojunctions are mainly affected not only by the diameter of the thinner segment of the SWCNT heterojunction but also by the orientation of the heptagon-heptagon (7-7) pair in the junction region. Moreover, the orientation of the 7-7 pair strongly affects those properties in the compression loading than those in tensile loading. Finally, it is found that the location of buckling deformation in the heterojunctions is dependent on the orientation of the 7-7 pair in the compression. (C) 2013 AIP Publishing LLC. C1 [Lee, Wen-Jay; Su, Wan-Sheng] Natl Ctr High Performance Comp, Taichung 40763, Taiwan. [Chang, Jee-Gong; Wang, Yeng-Tseng] Natl Ctr High Performance Comp, Tainan 74147, Taiwan. [Yang, An-Cheng] Natl Ctr High Performance Comp, Hsinchu 30076, Taiwan. [Wang, Yeng-Tseng] Kaohsiung Med Univ, Dept Biochem, Coll Med, Kaohsiung 80708, Taiwan. [Su, Wan-Sheng] Natl Chung Hsing Univ, Dept Phys, Taichung 40227, Taiwan. [Wang, Cai-Zhuang; Ho, Kai-Ming] Iowa State Univ, Ames Lab US DOE, Ames, IA 50011 USA. [Wang, Cai-Zhuang; Ho, Kai-Ming] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. RP Su, WS (reprint author), Natl Ctr High Performance Comp, Taichung 40763, Taiwan. EM wssu@nchc.narl.org.tw FU National Science Council (NSC) of Taiwan [NSC 102-2218-E-492-002, NSC-95-2917-I-194-010, NSC-101-2112-M-492-001-MY3]; US Department of Energy, Basic Energy Sciences, Division of Materials Science and Engineering [DE-AC02-07CH11358] FX The authors acknowledge the National Center for Theoretical Sciences (South) in Taiwan and financial support from the National Science Council (NSC) of Taiwan under Grant Nos. NSC 102-2218-E-492-002 (WJL), NSC-95-2917-I-194-010 (WSS), and NSC-101-2112-M-492-001-MY3 (WSS). Work at Ames Laboratory was supported by the US Department of Energy, Basic Energy Sciences, Division of Materials Science and Engineering, under Contract No. DE-AC02-07CH11358, including a grant of computer time at the National Energy Research Supercomputing Centre (NERSC) in Berkeley, CA. The authors are grateful to the National Center for High-performance Computing (NCHC) in providing huge computing resources to facilitate this research. NR 25 TC 1 Z9 1 U1 3 U2 22 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD OCT 14 PY 2013 VL 114 IS 14 AR 144306 DI 10.1063/1.4824539 PG 5 WC Physics, Applied SC Physics GA 236FI UT WOS:000325780400047 ER PT J AU Modine, NA Armstrong, AM Crawford, MH Chow, WW AF Modine, N. A. Armstrong, A. M. Crawford, M. H. Chow, W. W. TI Highly nonlinear defect-induced carrier recombination rates in semiconductors SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID LIGHT-EMITTING-DIODES; MULTIPHONON EMISSION; LUMINESCENCE; GAAS; GAP AB Defects in semiconductors can induce recombination of carriers and thus can strongly influence the efficiency and performance of solid-state devices. In the analysis of device performance, defect-induced recombination is often assumed to depend linearly on the carrier concentration or to be given by a sum of Shockley-Read-Hall expressions taken independently for each known defect level. Under these assumptions, defect-induced recombination increases with carrier concentration more slowly than both band-to-band radiative recombination and Auger recombination and becomes relatively less important at higher carrier concentrations. However, we show that defects with multiple defect levels can induce recombination with a highly nonlinear dependence on carrier concentration. For such defects, the usual assumptions about the relative importance of different recombination mechanisms at different carrier concentrations may fail. In order to demonstrate the potential impact of this phenomenon on realistic devices, we incorporate the defect-induced recombination rates obtained from our analysis into a microscopic InGaN/GaN light-emitting diode (LED) model. Our results indicate that a particular class of defects with plausible properties can induce a loss of optical efficiency at carrier concentrations relevant for high-power LED operation. (C) 2013 AIP Publishing LLC. C1 [Modine, N. A.; Armstrong, A. M.; Crawford, M. H.; Chow, W. W.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Modine, NA (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. FU Sandia's Solid-State Lighting Science Energy Frontier Research Center; Department of Energy Office of Basic Energy Science; United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported by Sandia's Solid-State Lighting Science Energy Frontier Research Center, sponsored by the Department of Energy Office of Basic Energy Science. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Company, for the United States Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL85000. NR 35 TC 5 Z9 5 U1 0 U2 21 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD OCT 14 PY 2013 VL 114 IS 14 AR 144502 DI 10.1063/1.4824065 PG 10 WC Physics, Applied SC Physics GA 236FI UT WOS:000325780400055 ER PT J AU Singh, DJ Parker, D AF Singh, David J. Parker, David TI Electronic and transport properties of zintl phase AeMg(2)Pn(2), Ae = Ca,Sr,Ba, Pn = As,Sb,Bi in relation to Mg3Sb2 SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID GENERALIZED GRADIENT APPROXIMATION; SOLIDS AB First principles calculations of the electronic structure and transport properties of Zintl phase AeMg(2)Pn(2), Ae = Ca,Sr,Ba, Pn = As,Sb,Bi compounds and Mg3Sb2 are reported. These are discussed in relation to the thermoelectric performance of the compounds and specifically the optimization of carrier concentration. It is found that there are several promising compositions and that the materials that have been studied to date are not fully optimized in terms of carrier concentration and may not ultimately be the best thermoelectrics in this family. We additionally report optical properties and show that there are significant differences among the compounds arising from differences in electronic structure and that these differences should be accessible to experiment. This provides a way to test the trends observed here. (C) 2013 AIP Publishing LLC. C1 [Singh, David J.; Parker, David] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Singh, DJ (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. NR 22 TC 9 Z9 9 U1 8 U2 54 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD OCT 14 PY 2013 VL 114 IS 14 AR 143703 DI 10.1063/1.4824465 PG 7 WC Physics, Applied SC Physics GA 236FI UT WOS:000325780400018 ER PT J AU Bowring, MA Bergman, RG Tilley, TD AF Bowring, Miriam A. Bergman, Robert G. Tilley, T. Don TI Isolation of a Dicationic Platinum Complex with Two Accessible Coordination Sites SO ORGANOMETALLICS LA English DT Article ID TRANSITION-METAL-COMPLEXES; H BOND ACTIVATION; PALLADIUM(II) COMPLEXES; CATIONIC PLATINUM(II); INTERNAL OLEFINS; CATALYSIS; ACID; HYDROAMINATION; NUCLEOPHILES; ETHYLENE AB The dicationic Pt complex [((t)Bu(2)bpy)Pt](NTf2)(2)center dot 1/2C(6)H(6) ((t)Bu(2)bpy = 4,4'-di-tert-butyl-2,2'-bipyridine, NTf2- = N(SO2CF3)(2)(-)) has been isolated and characterized. The new complex is supported by a simple bidentate bipyridine ligand and weakly coordinating, easily displaced triflimidate counterions. The Pt salt is competent for allylic C-H activation in aprotic, nonpolar media. C1 [Bergman, Robert G.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Bergman, RG (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM rbergman@berkeley.edu; tdtilley@berkeley.edu FU Office of Energy Research, Office of Basic Energy Sciences, Chemical Sciences Division, of the U.S. Department of Energy [DE-AC02-05CH11231] FX We gratefully acknowledge financial support from the Director of the Office of Energy Research, Office of Basic Energy Sciences, Chemical Sciences Division, of the U.S. Department of Energy under Contract DE-AC02-05CH11231. For technical assistance and helpful discussion, we thank Dr. Anthony T. Iavarone of the QB3/Chemistry Mass Spectrometry Facility and Dr. Antonio DiPasquale of the College of Chemistry X-ray Crystallography Facility, both at the University of California, Berkeley. For additional assistance with X-ray crystallography, we thank Michael I. Lipschutz. NR 28 TC 2 Z9 2 U1 1 U2 6 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0276-7333 EI 1520-6041 J9 ORGANOMETALLICS JI Organometallics PD OCT 14 PY 2013 VL 32 IS 19 BP 5266 EP 5268 DI 10.1021/om4009357 PG 3 WC Chemistry, Inorganic & Nuclear; Chemistry, Organic SC Chemistry GA 240UG UT WOS:000326122600007 ER PT J AU Nocton, G Booth, CH Maron, L Andersen, RA AF Nocton, Gregory Booth, Corwin H. Maron, Laurent Andersen, Richard A. TI Influence of the Torsion Angle in 3,3 '-Dimethyl-2,2 '-bipyridine on the Intermediate Valence of Yb in (C5Me5)(2)Yb(3,3 '-Me-2-bipy) SO ORGANOMETALLICS LA English DT Article ID DECAMETHYLYTTERBOCENE COMPLEXES; DIPERCHLORATE MONOHYDRATE; LANTHANIDE COMPLEXES; GROUND-STATE; BIPYRIDINES; 1,1'-BIISOQUINOLINE; COORDINATION; COVALENCY; EXCHANGE; OSMIUM AB The synthesis and X-ray crystal structures of Cp-2*Yb(3,3'-Me(2)bipy) and [Cp-2*Yb(3,3'-Me(2)bipy)][Cp-2*YbCl1.6I0.4]center dot CH2Cl2 are described. In both complexes, the NCCN torsion angles are approximately 40 degrees. The temperature-independent value of n(f) of 0.17 shows that the valence of ytterbium in the neutral adduct is multiconfigurational, in reasonable agreement with a CASSCF calculation that yields a n(f) value of 0.27; that is, the two configurations in the wave function are f(13)(pi(1)*)(1) and f(14)(pi(1)*)(0) in a ratio of 0.27:0.73, respectively, and the open-shell singlet lies 0.28 eV below the triplet state (n(f) accounts for f-hole occupancy; that is, n(f) = 1 when the configuration is f(13) and n(f) = 0 when the configuration is f(14)). A correlation is outlined between the value of nf and the individual ytterbocene and bipyridine fragments such that, as the reduction potentials of the ytterbocene cation and the free x,x'-R-2-bipy ligands approach each other, the value of nf and therefore the f(13):f(14) ratio reaches a maximum; conversely, the ratio is minimized as the disparity increases. C1 [Nocton, Gregory] Ecole Polytech, CNRS, Lab Heteroelements & Coordinat, F-91128 Palaiseau, France. [Nocton, Gregory; Andersen, Richard A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Booth, Corwin H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Maron, Laurent; Andersen, Richard A.] Univ Toulouse, CNRS, INSA, UPS,LPCNO,UMR 5215, Toulouse, France. RP Nocton, G (reprint author), Ecole Polytech, CNRS, Lab Heteroelements & Coordinat, Route Saclay, F-91128 Palaiseau, France. EM greg.nocton@polytechnique.edu; raandersen@lbl.gov RI Nocton, Greg/D-4435-2009 FU Office of Energy Research, Office of Basic Energy Sciences, Chemical Sciences Division, of the U.S. Department of Energy [DE-AC02-05CH11231] FX Work at the University of California, Berkeley, and at Lawrence Berkeley National Laboratory was supported by the Director, Office of Energy Research, Office of Basic Energy Sciences, Chemical Sciences Division, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. X-ray absorption data were collected at the Stanford Synchrotron Radiation Lightsource, a Directorate of SLAC National Accelerator Laboratory and an Office of Science User Facility operated for the U.S. Department of Energy Office of Science by Stanford University. We thank Wayne Lukens for several discussions on the Hubbard molecular model and Antonio DiPasquale at CHEXRAY Berkeley for his help with crystal structures. NR 45 TC 11 Z9 11 U1 1 U2 12 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0276-7333 EI 1520-6041 J9 ORGANOMETALLICS JI Organometallics PD OCT 14 PY 2013 VL 32 IS 19 BP 5305 EP 5312 DI 10.1021/om400528d PG 8 WC Chemistry, Inorganic & Nuclear; Chemistry, Organic SC Chemistry GA 240UG UT WOS:000326122600015 ER PT J AU Basar, G Kharzeev, DE Zahed, I AF Basar, Gokce Kharzeev, Dmitri E. Zahed, Ismail TI Chiral and Gravitational Anomalies on Fermi Surfaces SO PHYSICAL REVIEW LETTERS LA English DT Article ID DENSE QCD; TOPOLOGICAL INSULATORS; FINITE-TEMPERATURE; VIOLATION; FIELD; MODEL; SPIN AB A Fermi surface threaded by a Berry phase can be described by the Wess-Zumino-Witten term. After gauging, it produces a five-dimensional Chern-Simons term in the action. We show how this Chern-Simons term captures the essence of the Abelian, non-Abelian, and mixed gravitational anomalies in describing both in- and off-equilibrium phenomena. In particular, we derive a novel contribution to the chiral vortical effect that arises when a temperature gradient is present. We also discuss the issue of universality of the anomalous currents. C1 [Basar, Gokce; Kharzeev, Dmitri E.; Zahed, Ismail] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Kharzeev, Dmitri E.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. RP Basar, G (reprint author), SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. EM basar@tonic.physics.sunysb.edu; dmitri.kharzeev@stonybrook.edu; zahed@tonic.physics.sunysb.edu RI Basar, Gokce/O-6277-2016 FU U.S. Department of Energy [DE-FG-88ER40388, DE-AC02-98CH10886] FX We thank Hans Hansson, Misha Lublinsky, Michael Stone, Grigory Volovik, and Ho-Ung Yee for discussions. This work was supported by the U.S. Department of Energy under Contracts No. DE-FG-88ER40388 and No. DE-AC02-98CH10886. NR 64 TC 18 Z9 18 U1 0 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 14 PY 2013 VL 111 IS 16 AR 161601 DI 10.1103/PhysRevLett.111.161601 PG 5 WC Physics, Multidisciplinary SC Physics GA 240TG UT WOS:000326119300006 ER PT J AU Delgado, F Batista, CD Fernandez-Rossier, J AF Delgado, F. Batista, C. D. Fernandez-Rossier, J. TI Local Probe of Fractional Edge States of S=1 Heisenberg Spin Chains SO PHYSICAL REVIEW LETTERS LA English DT Article ID HALDANE-GAP; ANTIFERROMAGNETIC CHAIN; ANISOTROPY; EXCITATIONS; FIELD; MAGNETIZATION; STATISTICS; Y2BANIO5; DEFECTS; HEAT AB Spin chains are among the simplest physical systems in which electron-electron interactions induce novel states of matter. Here we propose to combine atomic scale engineering and spectroscopic capabilities of state of the art scanning tunnel microscopy to probe the fractionalized edge states of individual atomic scale S = 1 spin chains. These edge states arise from the topological order of the ground state in the Haldane phase. We also show that the Haldane gap and the spin-spin correlation length can be measured with the same technique. C1 [Delgado, F.; Fernandez-Rossier, J.] Int Iberian Nanotechnol Lab INL, P-4715310 Braga, Portugal. [Batista, C. D.] Los Alamos Natl Lab, Div Theoret, T4, Los Alamos, NM 87545 USA. [Batista, C. D.] Los Alamos Natl Lab, CNLS, Los Alamos, NM 87545 USA. RP Delgado, F (reprint author), Int Iberian Nanotechnol Lab INL, Ave Mestre Jose Veiga, P-4715310 Braga, Portugal. EM fernando.delgado@inl.int RI fernandez-rossier, joaquin/C-3910-2009; Delgado, Fernando/E-5790-2013; INL, Citations/K-3436-2015; Batista, Cristian/J-8008-2016 OI fernandez-rossier, joaquin/0000-0003-2297-0289; Delgado, Fernando/0000-0003-2180-5273; INL, Citations/0000-0002-3745-5100; FU MEC-Spain [FIS2010-21883-C02-01, FIS2009-08744, CONSOLIDER CSD2007-0010]; European Union; Generalitat Valenciana [Prometeo 2012-11]; NNSA of the U.S. DOE at LANL [DE-AC52-06NA25396]; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; NSF [PHY-1066293] FX This work has been financially supported by MEC-Spain (Grants No. FIS2010-21883-C02-01, No. FIS2009-08744, and No. CONSOLIDER CSD2007-0010), European Union as well as Generalitat Valenciana, Grant No. Prometeo 2012-11. This work was carried out under the auspices of the NNSA of the U.S. DOE at LANL under Contract No. DE-AC52-06NA25396, and was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. This Letter is based upon work supported in part by the NSF under Grant No. PHY-1066293 and the hospitality of the Aspen Center for Physics. NR 44 TC 6 Z9 6 U1 1 U2 21 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 14 PY 2013 VL 111 IS 16 AR 167201 DI 10.1103/PhysRevLett.111.167201 PG 5 WC Physics, Multidisciplinary SC Physics GA 240TG UT WOS:000326119300014 PM 24182294 ER PT J AU Bent, ZW Brazel, DM Tran-Gyamfi, MB Hamblin, RY VanderNoot, VA Branda, SS AF Bent, Zachary W. Brazel, David M. Tran-Gyamfi, Mary B. Hamblin, Rachelle Y. VanderNoot, Victoria A. Branda, Steven S. TI Use of a Capture-Based Pathogen Transcript Enrichment Strategy for RNA-Seq Analysis of the Francisella Tularensis LVS Transcriptome during Infection of Murine Macrophages SO PLOS ONE LA English DT Article ID LIVE VACCINE STRAIN; VIRULENCE GENE-EXPRESSION; ESCHERICHIA-COLI; INTRAMACROPHAGE GROWTH; INTRACELLULAR GROWTH; RESPIRATORY BURST; OXIDATIVE STRESS; PURINE AUXOTROPH; SUF OPERON; IDENTIFICATION AB Francisella tularensis is a zoonotic intracellular pathogen that is capable of causing potentially fatal human infections. Like all successful bacterial pathogens, F. tularensis rapidly responds to changes in its environment during infection of host cells, and upon encountering different microenvironments within those cells. This ability to appropriately respond to the challenges of infection requires rapid and global shifts in gene expression patterns. In this study, we use a novel pathogen transcript enrichment strategy and whole transcriptome sequencing (RNA-Seq) to perform a detailed characterization of the rapid and global shifts in F. tularensis LVS gene expression during infection of murine macrophages. We performed differential gene expression analysis on all bacterial genes at two key stages of infection: phagosomal escape, and cytosolic replication. By comparing the F. tularensis transcriptome at these two stages of infection to that of the bacteria grown in culture, we were able to identify sets of genes that are differentially expressed over the course of infection. This analysis revealed the temporally dynamic expression of a number of known and putative transcriptional regulators and virulence factors, providing insight into their role during infection. In addition, we identified several F. tularensis genes that are significantly up-regulated during infection but had not been previously identified as virulence factors. These unknown genes may make attractive therapeutic or vaccine targets. C1 [Bent, Zachary W.; Brazel, David M.; Tran-Gyamfi, Mary B.; Hamblin, Rachelle Y.; VanderNoot, Victoria A.; Branda, Steven S.] Sandia Natl Labs, Livermore, CA USA. RP Bent, ZW (reprint author), Sandia Natl Labs, Livermore, CA USA. EM zbent@sandia.gov OI Brazel, David/0000-0001-5361-2498 FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 69 TC 5 Z9 5 U1 1 U2 19 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD OCT 14 PY 2013 VL 8 IS 10 AR UNSP e77834 DI 10.1371/journal.pone.0077834 PG 12 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 237RD UT WOS:000325887300109 PM 24155975 ER PT J AU Bettencourt, LMA Trancik, JE Kaur, J AF Bettencourt, Luis M. A. Trancik, Jessika E. Kaur, Jasleen TI Determinants of the Pace of Global Innovation in Energy Technologies SO PLOS ONE LA English DT Article ID RESEARCH-AND-DEVELOPMENT; CLIMATE-CHANGE-MITIGATION; PATENTS; ELECTRICITY; INVESTMENT; KNOWLEDGE; INVENTION; PROGRESS; FUTURE; POLICY AB Understanding the factors driving innovation in energy technologies is of critical importance to mitigating climate change and addressing other energy-related global challenges. Low levels of innovation, measured in terms of energy patent filings, were noted in the 1980s and 90s as an issue of concern and were attributed to limited investment in public and private research and development (R&D). Here we build a comprehensive global database of energy patents covering the period 1970-2009, which is unique in its temporal and geographical scope. Analysis of the data reveals a recent, marked departure from historical trends. A sharp increase in rates of patenting has occurred over the last decade, particularly in renewable technologies, despite continued low levels of R&D funding. To solve the puzzle of fast innovation despite modest R&D increases, we develop a model that explains the nonlinear response observed in the empirical data of technological innovation to various types of investment. The model reveals a regular relationship between patents, R&D funding, and growing markets across technologies, and accurately predicts patenting rates at different stages of technological maturity and market development. We show quantitatively how growing markets have formed a vital complement to public R&D in driving innovative activity. These two forms of investment have each leveraged the effect of the other in driving patenting trends over long periods of time. C1 [Bettencourt, Luis M. A.; Trancik, Jessika E.] Santa Fe Inst, Santa Fe, NM 87501 USA. [Bettencourt, Luis M. A.] Los Alamos Natl Lab, Theoret Div T5, Los Alamos, NM USA. [Trancik, Jessika E.] MIT, Engn Syst Div, Cambridge, MA 02139 USA. [Kaur, Jasleen] Indiana Univ, Sch Informat & Comp, Ctr Complex Networks & Syst Res, Bloomington, IN USA. RP Trancik, JE (reprint author), Santa Fe Inst, Santa Fe, NM 87501 USA. EM trancik@mit.edu FU Army Research Office [W911NF-12-1-0097]; Los Alamos National Laboratory LDRD program [SGER-0742161]; National Science Foundation [SBE-0738187]; Solomon Buchsbaum Research Fund FX This work was supported by: the Army Research Office under grant W911NF-12-1-0097 (to LB); the Los Alamos National Laboratory LDRD program under grant SGER-0742161 (to LB); the National Science Foundation under grant SBE-0738187 (to JET); and the Solomon Buchsbaum Research Fund (to JET). The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 40 TC 17 Z9 17 U1 2 U2 19 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD OCT 14 PY 2013 VL 8 IS 10 AR e67864 DI 10.1371/journal.pone.0067864 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 237RD UT WOS:000325887300001 PM 24155867 ER PT J AU Hinckley, DM Freeman, GS Whitmer, JK de Pablo, JJ AF Hinckley, Daniel M. Freeman, Gordon S. Whitmer, Jonathan K. de Pablo, Juan J. TI An experimentally-informed coarse-grained 3-site-per-nucleotide model of DNA: Structure, thermodynamics, and dynamics of hybridization SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID SINGLE-STRANDED-DNA; MOLECULAR-DYNAMICS; NUCLEIC-ACIDS; MONTE-CARLO; SIMULATIONS; PROTEINS; WATER; KINETICS; CHAINS; IONS AB A new 3-Site-Per-Nucleotide coarse-grained model for DNA is presented. The model includes anisotropic potentials between bases involved in base stacking and base pair interactions that enable the description of relevant structural properties, including the major and minor grooves. In an improvement over available coarse-grained models, the correct persistence length is recovered for both ssDNA and dsDNA, allowing for simulation of non-canonical structures such as hairpins. DNA melting temperatures, measured for duplexes and hairpins by integrating over free energy surfaces generated using metadynamics simulations, are shown to be in quantitative agreement with experiment for a variety of sequences and conditions. Hybridization rate constants, calculated using forward-flux sampling, are also shown to be in good agreement with experiment. The coarse-grained model presented here is suitable for use in biological and engineering applications, including nucleosome positioning and DNA-templated engineering. (C) 2013 AIP Publishing LLC. C1 [Hinckley, Daniel M.; Freeman, Gordon S.] Univ Wisconsin, Dept Chem & Biol Engn, Madison, WI 53706 USA. [Whitmer, Jonathan K.; de Pablo, Juan J.] Argonne Natl Lab, Inst Mol Engn, Argonne, IL 60439 USA. [de Pablo, Juan J.] Univ Chicago, Inst Mol Engn, Chicago, IL 60637 USA. RP Hinckley, DM (reprint author), Univ Wisconsin, Dept Chem & Biol Engn, Madison, WI 53706 USA. EM depablo@uchicago.edu FU National Science Foundation (NSF); NSF through the University of Wisconsin-Madison Nanoscale Science and Engineering Center [DMR0832760]; [T32HG002760] FX The authors thank Dr. Gregory N. Toepperwein for helpful discussions. The University of Wisconsin-Madison Center for High Throughput Computing is gratefully acknowledged for providing resources and computer expertise. D. M. H., G. S. F., and J.K.W. were funded in part through Training Grant T32HG002760 to the Genomic Sciences Training Program. D. M. H. was also supported by a Graduate Research Fellowship from the National Science Foundation (NSF). This work was supported by the NSF through the University of Wisconsin-Madison Nanoscale Science and Engineering Center (Grant No. DMR0832760). We also thank anonymous referees whose comments led to significant improvements to this paper. NR 81 TC 45 Z9 45 U1 4 U2 45 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD OCT 14 PY 2013 VL 139 IS 14 AR 144903 DI 10.1063/1.4822042 PG 16 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 236FL UT WOS:000325780800049 PM 24116642 ER PT J AU Kim, SY Perez, D Voter, AF AF Kim, Soo Young Perez, Danny Voter, Arthur F. TI Local hyperdynamics SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID ACCELERATED MOLECULAR-DYNAMICS; INFREQUENT EVENTS; BOOST METHOD; TIME-SCALE; SIMULATION; DIFFUSION; SURFACES AB We present a new formulation of the hyperdynamics method in which the biasing effect is local, making it suitable for large systems. In standard hyperdynamics, the requirement that the bias potential be zero everywhere on the dividing surface bounding the state has the consequence that as the system size increases the boost factor decays to unity, regardless of the form of the bias potential. In the new method, the bias force on each atom is obtained by differentiating a local bias energy that depends only on the coordinates of atoms within a finite range of this atom. This bias force is thus independent of the bias force in distant parts of the system, providing a method that gives a constant boost factor, independent of the system size. We demonstrate for some realistic atomistic systems that the method gives escape rates in excellent agreement with direct molecular dynamics simulations. (C) 2013 AIP Publishing LLC. C1 [Kim, Soo Young; Perez, Danny; Voter, Arthur F.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Kim, SY (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. OI Voter, Arthur/0000-0001-9788-7194 FU Laboratory Directed Research and Development (LDRD) program at Los Alamos National Laboratory (LANL); United States Department of Energy (U.S. DOE), Office of Basic Energy Sciences, Materials Sciences and Engineering Division; National Nuclear Security Administration of the U.S. DOE [DE-AC52-O6NA25396] FX We are grateful to R. A. Miron for the suggestion that initiated this research project, and to T. C. Germann, Shiyu Du, and Noam Bernstein for helpful discussions. This work was primarily supported by the Laboratory Directed Research and Development (LDRD) program at Los Alamos National Laboratory (LANL). It was also supported in the early and late stages by the United States Department of Energy (U. S. DOE), Office of Basic Energy Sciences, Materials Sciences and Engineering Division. LANL is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. DOE, under Contract No. DE-AC52-O6NA25396. NR 34 TC 8 Z9 8 U1 2 U2 26 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD OCT 14 PY 2013 VL 139 IS 14 AR 144110 DI 10.1063/1.4824389 PG 14 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 236FL UT WOS:000325780800013 PM 24116606 ER PT J AU Ou, YP Sokoloff, JB Stevens, MJ AF Ou, Yangpeng Sokoloff, Jeffrey B. Stevens, Mark J. TI Discrete model studies of two grafted polyelectrolyte polymer hydrogels pressed in contact SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID MOLECULAR-DYNAMICS SIMULATION; MONTE-CARLO-SIMULATION; MECHANICAL-PROPERTIES; GELS; NETWORKS; FRICTION; TRANSITIONS; SURFACES; BRUSHES; SYSTEMS AB The interaction between two grafted polymer gels was investigated. We studied a defect-free network of diamond-like topology containing 8 tetra-functional nodes linked by 16 non-crossing chains. In order to explain the very low friction coefficient observed for polyelectrolyte hydrogels, we computed the monomer density profile of these polymer gels, the interpenetration between two polymer gels (defined as the percentage of monomers belonging to one gel which have penetrated the second gel), the normal force per unit area, and the radial distribution function of the interacting monomers. Low monomer density in the interface region separating the two gels and low interpenetration of the gels similar to that found in our simulations are likely to be responsible for the small friction coefficients observed for polyelectrolyte polymer gels. (C) 2013 AIP Publishing LLC. C1 [Ou, Yangpeng; Sokoloff, Jeffrey B.] Northeastern Univ, Dept Phys, Boston, MA 02115 USA. [Ou, Yangpeng; Sokoloff, Jeffrey B.] Northeastern Univ, Ctr Interdisciplinary Res Complex Syst, Boston, MA 02115 USA. [Stevens, Mark J.] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA. RP Ou, YP (reprint author), Northeastern Univ, Dept Phys, Boston, MA 02115 USA. EM ou.y@outlook.com OI Sokoloff, Jeffrey/0000-0002-6124-8056 FU United States Department of Energy [DE-AC04-94AL85000]; U.S. Department of Energy, Center for Integrated Nanotechnologies, at Los Alamos National Laboratory [DE-AC52-06NA25396]; Sandia National Laboratories FX Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy under Contract No. DE-AC04-94AL85000. This work was performed at the U.S. Department of Energy, Center for Integrated Nanotechnologies, at Los Alamos National Laboratory (Contract No. DE-AC52-06NA25396) and Sandia National Laboratories. NR 40 TC 2 Z9 2 U1 0 U2 8 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD OCT 14 PY 2013 VL 139 IS 14 AR 144902 DI 10.1063/1.4823773 PG 5 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 236FL UT WOS:000325780800048 PM 24116641 ER PT J AU Weichman, ML Kim, JB Neumark, DM AF Weichman, Marissa L. Kim, Jongjin B. Neumark, Daniel M. TI Vibrational fine structure of C-5 via anion slow photoelectron velocity-map imaging SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID SMALL CARBON CLUSTERS; ELECTRONIC-ABSORPTION-SPECTRA; EMISSION PUMPING SPECTROSCOPY; AB-INITIO; NEON MATRICES; PHOTODETACHMENT SPECTROSCOPY; INFRARED-SPECTRUM; C-2N+1(-) N=2-5; OPTICAL-SPECTRA; LARGE MOLECULES AB High-resolution anion photoelectron spectra of cryogenically cooled C-5(-) clusters are reported using slow photoelectron velocity-map imaging spectroscopy. We resolve vibronic transitions to the nu(2) stretching mode and multiply excited nu(5), nu(6), and nu(7) bending modes of neutral C-5 with significantly higher accuracy than previous experiments. Weak transitions to Franck-Condon (FC) forbidden singly excited bending modes are made possible by Herzberg-Teller coupling between electronic states of the neutral cluster. In addition, we resolve vibrational fine structure corresponding to different angular momentum states of multiply excited bending modes. The observation of this multiplet structure, some of which is FC forbidden, is attributed to Renner-Teller coupling between vibrational levels in the C-5(-) ground electronic state. (C) 2013 AIP Publishing LLC. C1 [Weichman, Marissa L.; Kim, Jongjin B.; Neumark, Daniel M.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Neumark, Daniel M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Neumark, DM (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM dneumark@berkeley.edu RI Neumark, Daniel/B-9551-2009; OI Neumark, Daniel/0000-0002-3762-9473; Weichman, Marissa/0000-0002-2551-9146 FU Air Force Office of Scientific Research [FA9550-12-1-0160]; Defense University Research Instrumentation Program [FA9550-11-1-0300]; National Science Foundation FX This research is funded by the Air Force Office of Scientific Research under Grant No. FA9550-12-1-0160 and the Defense University Research Instrumentation Program under Grant No. FA9550-11-1-0300. M. L. W. thanks the National Science Foundation for a graduate research fellowship. NR 77 TC 4 Z9 4 U1 0 U2 23 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD OCT 14 PY 2013 VL 139 IS 14 AR 144314 DI 10.1063/1.4824657 PG 7 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 236FL UT WOS:000325780800033 PM 24116626 ER PT J AU Atalla, V Yoon, M Caruso, F Rinke, P Scheffler, M AF Atalla, Viktor Yoon, Mina Caruso, Fabio Rinke, Patrick Scheffler, Matthias TI Hybrid density functional theory meets quasiparticle calculations: A consistent electronic structure approach SO PHYSICAL REVIEW B LA English DT Article ID GW APPROXIMATION; EXACT-EXCHANGE; PHOTOELECTRON; POTENTIALS; INTERFACES; CHARGE; MODEL; TCNQ; GAS AB We propose a scheme to obtain a system-dependent fraction of exact exchange (alpha) within the framework of hybrid density functional theory (DFT) that is consistent with the G(0)W(0) approach, where G(0) is the noninteracting Green function of the system and W-0 the screened Coulomb interaction. We exploit the formally exact condition of exact DFT that the energy of the highest occupied molecular orbital corresponds to the ionization potential of a finite system. We identify the optimal alpha value for which this statement is obeyed as closely as possible and thereby remove the starting point dependence from the G(0)W(0) method. This combined approach is essential for describing electron transfer (as exemplified by the TTF/TCNQ dimer) and yields the vertical ionization potentials of the G2 benchmark set with a mean absolute percentage error of only approximate to 3%. C1 [Atalla, Viktor; Caruso, Fabio; Rinke, Patrick; Scheffler, Matthias] Max Planck Gesell, Fritz Haber Inst, D-14195 Berlin, Germany. [Atalla, Viktor; Yoon, Mina] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Atalla, V (reprint author), Max Planck Gesell, Fritz Haber Inst, Faradayweg 4-6, D-14195 Berlin, Germany. EM atalla@fhi-berlin.mpg.de RI Rinke, Patrick/A-4208-2010; Caruso, Fabio/D-5917-2013; Yoon, Mina/A-1965-2016; Scheffler, Matthias/O-4649-2016 OI Rinke, Patrick/0000-0002-5967-9965; Yoon, Mina/0000-0002-1317-3301; FU Laboratory Directed Research and Development award from Oak Ridge National Laboratory (ORNL); Scientific User Facilities Division at the Center for Nanophase Materials Sciences at ORNL by the Office of Basic Energy Sciences, US Department of Energy; National Energy Research Scientific Computing Center [DE-AC02-05CH11231] FX V.A. acknowledges partial support provided by a Laboratory Directed Research and Development award from Oak Ridge National Laboratory (ORNL). M.Y. was supported by the Scientific User Facilities Division at the Center for Nanophase Materials Sciences at ORNL by the Office of Basic Energy Sciences, US Department of Energy, and National Energy Research Scientific Computing Center under Contract No. DE-AC02-05CH11231. NR 46 TC 50 Z9 50 U1 3 U2 43 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 14 PY 2013 VL 88 IS 16 AR 165122 DI 10.1103/PhysRevB.88.165122 PG 8 WC Physics, Condensed Matter SC Physics GA 233KD UT WOS:000325566300002 ER PT J AU Chyzh, A Wu, CY Kwan, E Henderson, RA Gostic, JM Bredeweg, TA Couture, A Haight, RC Lee, HY O'Donnell, JM Ullmann, JL AF Chyzh, A. Wu, C. Y. Kwan, E. Henderson, R. A. Gostic, J. M. Bredeweg, T. A. Couture, A. Haight, R. C. Lee, H. Y. O'Donnell, J. M. Ullmann, J. L. TI Precision measurement of the Pu-238(n, gamma) cross section SO PHYSICAL REVIEW C LA English DT Article ID NUCLEAR-DATA; NEUTRON; TECHNOLOGY; SCIENCE AB The neutron-capture cross section for Pu-238 was measured by using the detector for advanced neutron-capture experiments (DANCE) array, which is a highly segmented and highly efficient 4 pi gamma-ray calorimeter. The neutron-capture events were recognized by the total gamma-ray energy deposited in DANCE, which is equal to the reaction Q value plus the incident neutron energy. The absolute neutron-capture cross section was derived as a function of incident neutron energy from thermal to about 30 keV. The measured cross section for incident neutron energy below 18 eV was performed for the first time by using the direct method and does not support the most recently adopted changes in ENDF/B-VII.1 where the neutron-capture cross section was lowered by as much as a factor of similar to 3 in the neighborhood of 0.3 eV from those evaluated in ENDF/B-VII.0. C1 [Chyzh, A.; Wu, C. Y.; Kwan, E.; Henderson, R. A.; Gostic, J. M.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Bredeweg, T. A.; Couture, A.; Haight, R. C.; Lee, H. Y.; O'Donnell, J. M.; Ullmann, J. L.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Kwan, E.] Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA. RP Chyzh, A (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. FU U.S. Department of Energy by Lawrence Livermore National Security, LLC [DE-AC52-07NA27344]; Los Alamos National Security, LLC [DE-AC52-06NA25396]; U.S. DOE/NNSA Office of Defense Nuclear Nonproliferation Research and Development FX We thank Dr. P. Koehler for a very helpful discussion on various issues related to SAMMY in extracting the resonance width. This work benefited from the use of the LANSCE accelerator facility as performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Security, LLC under Contract No. DE-AC52-07NA27344 and by Los Alamos National Security, LLC under Contract No. DE-AC52-06NA25396. Partial funding is gratefully acknowledged from the U.S. DOE/NNSA Office of Defense Nuclear Nonproliferation Research and Development. The 238Pu isotope used in the measurements was obtained from Oak Ridge National Laboratory. NR 20 TC 2 Z9 2 U1 0 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD OCT 14 PY 2013 VL 88 IS 4 AR 044607 DI 10.1103/PhysRevC.88.044607 PG 5 WC Physics, Nuclear SC Physics GA 233QC UT WOS:000325583100005 ER PT J AU Czerwinski, M Razca-Urban, T Sieja, K Sliwinska, H Urban, W Smith, AG Smith, JF Simpson, GS Ahmad, I Greene, JP Materna, T AF Czerwinski, M. Razca-Urban, T. Sieja, K. Sliwinska, H. Urban, W. Smith, A. G. Smith, J. F. Simpson, G. S. Ahmad, I. Greene, J. P. Materna, T. TI Yrast excitations in the neutron-rich N=52 isotones SO PHYSICAL REVIEW C LA English DT Article ID NUCLEAR-DATA SHEETS; SHELL-MODEL; FISSION FRAGMENTS; SHAPE TRANSITION; LARGE ARRAYS; DEFORMATION; DETECTORS; ISOTOPES; STATES AB The Kr-88 nucleus has been reinvestigated with prompt-gamma-ray-spectroscopy methods using the Gammasphere Ge array to measure gamma rays following spontaneous fission of Cf-252. The order of some of the transitions, reported previously, has been changed and new levels were introduced. Angular correlation analysis allowed the assignment of spins to several levels in Kr-88. These data, together with the shell-model calculations, explained the near-yrast structure of Kr-88, which is similar to the structure of the N = 52, Sr-90, and Zr-92 isotones. The regular systematics obtained for the three isotones suggests that the spin of the 2073.4-keV level in the Se-86 isotone is different from the I = 6 value reported previously. Using data from prompt gamma-ray measurement of spontaneous fission of Cm-248, we reinvestigated the 86Se nucleus. A new candidate for the 6(1)(+) level in Se-86 has been proposed, which is supported by shell-model calculations. Energies of the 2(1)(+) and 4(1)(+) levels in the Zn-82 nucleus have been predicted using a novel systematics. C1 [Czerwinski, M.; Razca-Urban, T.; Urban, W.] Univ Warsaw, Fac Phys, PL-00681 Warsaw, Poland. [Sieja, K.; Sliwinska, H.] Univ Strasbourg, IPHC, F-67037 Strasbourg, France. [Sieja, K.; Sliwinska, H.] CNRS, UMR7178, F-67037 Strasbourg, France. [Urban, W.] Inst Laue Langevin, F-38042 Grenoble 9, France. [Smith, A. G.; Smith, J. F.] Univ Manchester, Dept Phys & Astron, Manchester M13 9PL, Lancs, England. [Simpson, G. S.] Univ Grenoble 1, LPSC, CNRS IN2P3, Inst Natl Polytech Grenoble, F-38026 Grenoble, France. [Ahmad, I.; Greene, J. P.] Argonne Natl Lab, Argonne, IL 60439 USA. [Materna, T.] CEA Saclay, IRFU SPHN, F-91191 Gif Sur Yvette, France. RP Czerwinski, M (reprint author), Univ Warsaw, Fac Phys, Hoza 69, PL-00681 Warsaw, Poland. EM teresa.rzaca@fuw.edu.pl FU US Department of Energy, Office of Nuclear Physics [DE-AC02-06CH11357] FX The authors would like to thank M. P. Carpenter, R. V. F. Janssens, F. G. Kondev, T. Lauritsen, C. J. Lister, and D. Seweryniak of the Physics Division of Argonne National Laboratory for their help in preparing and running the Gammasphere measurement. This work was partially supported by the US Department of Energy, Office of Nuclear Physics, under Contract No. DE-AC02-06CH11357. The authors are indebted for the use of 248Cm to the Office of Basic Energy Sciences, Department of Energy, through the transplutonium element production facilities at Oak Ridge National Laboratory. NR 42 TC 16 Z9 16 U1 1 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD OCT 14 PY 2013 VL 88 IS 4 AR 044314 DI 10.1103/PhysRevC.88.044314 PG 13 WC Physics, Nuclear SC Physics GA 233QC UT WOS:000325583100002 ER PT J AU Miernik, K AF Miernik, K. TI Phenomenological model of beta-delayed neutron-emission probability SO PHYSICAL REVIEW C LA English DT Article ID GROSS THEORY; DECAY; PRECURSORS; NUCLEUS AB A phenomenological model of the beta-delayed neutron-emission probability, based on a level density function, is presented. The effective level density systematics, empirically determined from the experimental data, are found to be relatively flat, with discontinuities at the major shell closures. These systematics have been modeled and used to determine beta-delayed neutron-emission probabilities. The present model is compared to other available models and is found to provide an improved description of the beta-delayed neutron-emission probabilities across the entire mass surface. C1 [Miernik, K.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37830 USA. [Miernik, K.] Univ Warsaw, Fac Phys, PL-00681 Warsaw, Poland. RP Miernik, K (reprint author), Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37830 USA. EM kmiernik@fuw.edu.pl FU Office of Nuclear Physics, US Department of Energy [DE-AC05-00OR22725]; UT-Battelle, LLC. FX The author thanks J. M. Allmond, R. Grzywacz, C. J. Gross, and K. P. Rykaczewski for valuable comments and discussions. This research is sponsored by the Office of Nuclear Physics, US Department of Energy under Contract No. DE-AC05-00OR22725 with UT-Battelle, LLC. NR 23 TC 10 Z9 10 U1 0 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD OCT 14 PY 2013 VL 88 IS 4 AR 041301 DI 10.1103/PhysRevC.88.041301 PG 4 WC Physics, Nuclear SC Physics GA 233QC UT WOS:000325583100001 ER PT J AU Harnik, R Martin, A Okui, T Primulando, R Yu, F AF Harnik, Roni Martin, Adam Okui, Takemichi Primulando, Reinard Yu, Felix TI Measuring CP violation in h -> tau(+)tau(-) at colliders SO PHYSICAL REVIEW D LA English DT Article ID HIGGS-BOSON; DECAY MODE; TAU; PARITY; MASS; LHC; TAUBARTAU AB We investigate the LHC and Higgs factory prospects for measuring the CP phase in the Higgs-tau-tau coupling. Currently this phase can be anywhere between 0 degrees (CP even) and 90 degrees (CP odd). A new, ideal observable is identified from an analytic calculation for the tau(+/-) -> rho(+/-)nu -> pi(+/-)pi(0)nu channel. It is demonstrated to have promising sensitivity at the LHC and superior sensitivity at the ILC compared to previous proposals. Our observable requires the reconstruction of the internal substructure of decaying taus but does not rely on measuring the impact parameter of tau decays. It is the first proposal for such a measurement at the LHC. For the 14 TeV LHC, we estimate that about 1 ab(-1) data can discriminate CP even versus CP odd at the 5 sigma level. With 3 ab(-1), the CP phase should be measurable to an accuracy of similar to 11 degrees. At an e(+)e(-) Higgs factory, we project that a 250 GeV run with 1 ab(-1) luminosity can measure the phase to similar to 4.4 degrees accuracy. C1 [Harnik, Roni; Yu, Felix] Fermilab Natl Accelerator Lab, Dept Theoret Phys, Batavia, IL 60510 USA. [Martin, Adam] Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. [Martin, Adam] CERN, PH TH Dept, CH-1211 Geneva 23, Switzerland. [Okui, Takemichi] Florida State Univ, Dept Phys, Tallahassee, FL 32306 USA. [Primulando, Reinard] Johns Hopkins Univ, Dept Phys & Astron, Baltimore, MD 21218 USA. RP Harnik, R (reprint author), Fermilab Natl Accelerator Lab, Dept Theoret Phys, POB 500, Batavia, IL 60510 USA. FU NSF [PHY-0910467]; DOE [DE-FG02-13ER41942]; United States Department of Energy [De-AC02-07CH11359] FX We would like to thank Kaustubh Agashe, Wolfgang Altmannshofer, Yuval Grossman, Uli Haisch, Josh Ruderman, Daniel Stolarski, Raman Sundrum, Ciaran Williams, and Jure Zupan for comments and discussions. We would also like to thank the Kavli Institute for Theoretical Physics at UCSB where part of this work was performed. R. P. is supported by the NSF under Grant No. PHY-0910467. T. O. is supported by the DOE under Grant No. DE-FG02-13ER41942. Fermilab is operated by the Fermi Research Alliance, LLC under Contract No. De-AC02-07CH11359 with the United States Department of Energy. NR 37 TC 26 Z9 26 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD OCT 14 PY 2013 VL 88 IS 7 AR 076009 DI 10.1103/PhysRevD.88.076009 PG 12 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 239RG UT WOS:000326042500008 ER PT J AU Reichhardt, C Reichhardt, CJO AF Reichhardt, C. Reichhardt, C. J. Olson TI Dynamics and separation of circularly moving particles in asymmetrically patterned arrays SO PHYSICAL REVIEW E LA English DT Article ID LOW-REYNOLDS-NUMBER; SWIMMING BACTERIA; MICROSWIMMERS; RATCHETS; MOTORS AB There are many examples of driven and active matter systems containing particles that exhibit circular motion with different chiralities, such as swimming bacteria near surfaces or certain types of self-driven colloidal particles. Circular motion of passive particles can also be induced with an external rotating drive. Here we examine particles that move in circles and interact with a periodic array of asymmetric L-shaped obstacles. We find a series of dynamical phases as a function of swimming radius, including regimes where the particle motion is rectified, producing a net dc motion. The direction of the rectification varies with the swimming radius, permitting the separation of particles with different swimming radii. Particles with the same swimming radius but different chirality can also move in different directions over the substrate and be separated. The rectification occurs for specific windows of swimming radii corresponding to periodic orbits in which the particles interact one or more times with the barriers per rotation cycle. The rectification effects are robust against the addition of thermal or diffusive effects, and are in some cases even enhanced by these effects. C1 [Reichhardt, C.; Reichhardt, C. J. Olson] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Reichhardt, C (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. OI Reichhardt, Cynthia/0000-0002-3487-5089 FU NNSA of the U.S. DoE at LANL [DE-AC52-06NA25396] FX We thank J. Drocco for useful discussions. This work was carried out under the auspices of the NNSA of the U.S. DoE at LANL under Contract No. DE-AC52-06NA25396. NR 44 TC 16 Z9 16 U1 1 U2 23 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD OCT 14 PY 2013 VL 88 IS 4 AR 042306 DI 10.1103/PhysRevE.88.042306 PG 10 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA 239TG UT WOS:000326047800008 PM 24229171 ER PT J AU Galan, BR Reback, ML Jain, A Appel, AM Shaw, WJ AF Galan, Brandon R. Reback, Matthew L. Jain, Avijita Appel, Aaron M. Shaw, Wendy J. TI Electrocatalytic Oxidation of Formate with Nickel Diphosphine Dipeptide Complexes: Effect of Ligands Modified with Amino Acids SO EUROPEAN JOURNAL OF INORGANIC CHEMISTRY LA English DT Article DE Formate; Oxidation; Nickel; Peptide catalysts; Electrocatalysts; Outer coordination sphere; Biocatalysts; Bioinorganic chemistry ID OUTER-COORDINATION SPHERE; FUEL-CELLS; CATALYSTS; TEMPERATURE AB A series of nickel bis(diphosphine) complexes with dipeptides appended to the ligands were investigated for the catalytic oxidation of formate to carbon dioxide, a proton, and two electrons. Typical rates of approximately 7 s(-1) were found, similar to that for the parent complex (ca. 8 s(-1)), with amino acid size and positioning contributing very little to the rate or operating potential. Hydroxy functionalities did result in lower rates, which were recovered by protecting the hydroxy group. The results suggest that the overall dielectric properties introduced by the dipeptides do not play an important role in catalysis, but free hydroxy groups do influence activity, implying contributions from intra- or intermolecular interactions. These observations are important in developing a fundamental understanding of the effect that an enzyme-like outer coordination sphere can have upon molecular catalysts. C1 [Galan, Brandon R.; Reback, Matthew L.; Jain, Avijita; Appel, Aaron M.; Shaw, Wendy J.] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. RP Appel, AM (reprint author), Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. EM aaron.appel@pnnl.gov; wendy.shaw@pnnl.gov OI Appel, Aaron/0000-0002-5604-1253 FU US Department of Energy (DOE) Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences Biosciences FX This work was funded by the US Department of Energy (DOE) Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences & Biosciences. Pacific Northwest National Laboratory (PNNL) is a multiprogram national laboratory operated for DOE by Battelle. NR 31 TC 5 Z9 5 U1 1 U2 17 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1434-1948 EI 1099-0682 J9 EUR J INORG CHEM JI Eur. J. Inorg. Chem. PD OCT 14 PY 2013 VL 2013 IS 30 BP 5366 EP 5371 DI 10.1002/ejic.201300751 PG 6 WC Chemistry, Inorganic & Nuclear SC Chemistry GA 233FC UT WOS:000325550800022 ER PT J AU Herklotz, A Kataja, M Nenkov, K Biegalski, MD Christen, HM Deneke, C Schultz, L Dorr, K AF Herklotz, A. Kataja, M. Nenkov, K. Biegalski, M. D. Christen, H. -M. Deneke, C. Schultz, L. Doerr, K. TI Magnetism of the tensile-strain-induced tetragonal state of SrRuO3 films SO PHYSICAL REVIEW B LA English DT Article ID THIN-FILMS; ELECTRONIC-STRUCTURE; MAGNETIZATION; TEMPERATURE; SUBSTRATE; GROWTH AB SrRuO3 films have been grown in the tetragonal, structurally single-domain state under 1% of biaxial tensile strain. The angular dependencies of the magnetization and the magnetoresistance reveal an upright orientation of the tetragonal unit cell and biaxial magnetic in-plane anisotropy with 110(t) easy axes. Reversible biaxial strain from piezoelectric Pb(Mg1/3Nb2/3)(0.72)Ti0.28O3 (PMN-PT) substrates has been applied to probe the direct strain response of the magnetization and the electrical resistance. At 1% tensile strain, the Curie temperature (T-C) and the ordered magnetic moment (m(S)) at low temperatures are found to substantially decrease with further growing tensile strain. This suggests a suppression of m(S) resulting from distortions of the RuO6 octahedra, in line with reported density-functional calculations. Reversible strain has also been applied to a film under weak tensile strain revealing the opposite response, i.e., an enhancement of T-C and m(S) with tensile strain. Structural and magnetic properties of SrRuO3 films in several static strain states (compressive, weak and strong tensile strain) are compared. C1 [Herklotz, A.; Doerr, K.] Univ Halle Wittenberg, Inst Phys, D-06120 Halle, Germany. [Herklotz, A.; Kataja, M.; Nenkov, K.; Schultz, L.] IFW Dresden, Inst Metall Mat, D-01069 Dresden, Germany. [Biegalski, M. D.; Christen, H. -M.] ORNL, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Deneke, C.] Lab Nacl Nanotecnol, BR-13083100 Campinas, SP, Brazil. RP Herklotz, A (reprint author), Univ Halle Wittenberg, Inst Phys, Von Danckelmann Pl 3, D-06120 Halle, Germany. RI Schultz, Ludwig/B-3383-2010; Christen, Hans/H-6551-2013; Deneke, Christoph/C-6828-2008; Kataja, Mikko/N-1683-2016 OI Christen, Hans/0000-0001-8187-7469; Deneke, Christoph/0000-0002-8556-386X; FU DFG [FOR520]; Scientific User Facilities Division, Office of Basic Energy Sciences, US DOE FX The authors would like to acknowledge the support of DFG FOR520 and the Scientific User Facilities Division, Office of Basic Energy Sciences, US DOE. We thank A. Malachias for assistance at the Brazilian National Synchrotron Light Laboratory-LNLS. NR 30 TC 10 Z9 10 U1 1 U2 55 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 14 PY 2013 VL 88 IS 14 AR 144412 DI 10.1103/PhysRevB.88.144412 PG 8 WC Physics, Condensed Matter SC Physics GA 233GT UT WOS:000325556900004 ER PT J AU Skinner, B Yu, GL Kretinin, AV Geim, AK Novoselov, KS Shklovskii, BI AF Skinner, Brian Yu, G. L. Kretinin, A. V. Geim, A. K. Novoselov, K. S. Shklovskii, B. I. TI Effect of dielectric response on the quantum capacitance of graphene in a strong magnetic field SO PHYSICAL REVIEW B LA English DT Article ID 2-DIMENSIONAL ELECTRON-GAS; METAL-INSULATOR-TRANSITION; DENSITY; SYSTEMS; COMPRESSIBILITY; ENERGY; LIQUID; STATES AB The quantum capacitance of graphene can be negative when the graphene is placed in a strong magnetic field, which is a clear experimental signature of positional correlations between electrons. Here we show that the quantum capacitance of graphene is also strongly affected by its dielectric polarizability, which in a magnetic field is wave-vector dependent. We study this effect both theoretically and experimentally. We develop a theory and numerical procedure for accounting for the graphene dielectric response, and we present measurements of the quantum capacitance of high-quality graphene capacitors on boron nitride. Theory and experiment are found to be in good agreement. C1 [Skinner, Brian; Shklovskii, B. I.] Univ Minnesota, Fine Theoret Phys Inst, Minneapolis, MN 55455 USA. [Skinner, Brian] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Yu, G. L.; Kretinin, A. V.; Geim, A. K.; Novoselov, K. S.] Univ Manchester, Sch Phys & Astron, Manchester M13 9PL, Lancs, England. RP Skinner, B (reprint author), Univ Minnesota, Fine Theoret Phys Inst, Minneapolis, MN 55455 USA. RI Kretinin, Andrey/L-5122-2013; Geim, Andre/J-7888-2012; Novoselov, Kostya/G-9581-2014 OI Skinner, Brian/0000-0003-0774-3563; Geim, Andre/0000-0003-2861-8331; Novoselov, Kostya/0000-0003-4972-5371 FU National Science Foundation through the University of Minnesota MRSEC [DMR-0819885]; NSF [1066293]; US Department of Energy, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX We are grateful to B. Feldman, M. M. Fogler, A. M. Straub, and A. Yacoby for helpful discussions. This work was supported primarily by the National Science Foundation through the University of Minnesota MRSEC under Award No DMR-0819885. B.S. and B.I.S. thank the Aspen Center for Physics for their hospitality, and acknowledge their NSF Grant No. 1066293. Work at Argonne National Laboratory was supported by the US Department of Energy, Office of Basic Energy Sciences under Contract No. DE-AC02-06CH11357. NR 55 TC 11 Z9 11 U1 3 U2 45 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 14 PY 2013 VL 88 IS 15 AR 155417 DI 10.1103/PhysRevB.88.155417 PG 9 WC Physics, Condensed Matter SC Physics GA 233IZ UT WOS:000325563200008 ER PT J AU Velarde, L Wang, HF AF Velarde, Luis Wang, Hong-fei TI Unique determination of the -CN group tilt angle in Langmuir monolayers using sum-frequency polarization null angle and phase SO CHEMICAL PHYSICS LETTERS LA English DT Article ID GENERATION VIBRATIONAL SPECTROSCOPY; AIR-WATER-INTERFACE; SURFACE 2ND-HARMONIC GENERATION; LIQUID-CRYSTAL; SFG-VS; MOLECULAR-ORIENTATION; FILMS; CONFORMATION; TRANSITIONS; METHYLENE AB The relative phase and amplitude ratio between the ssp and ppp polarization combinations of the vibrational sum-frequency generation (SFG) response can be uniquely and accurately determined by the polarization null angle (PNA) method for orientational analysis. With PNA measurement we show that the -CN group in the 4-n-pentyl-4'-cyanoterphenyl (5CT) Langmuir monolayer is tilted around 25 degrees +/- 2 degrees from the interface normal, while that in the 4-n-octyl-4'-cyanobiphenyl (8CB) is tilted around 57 degrees +/- 2 degrees, consistent with the significant differences in the phase diagrams and hydrogen bonding SFG spectra of the two Langmuir monolayers reported in the literature. (C) 2013 Elsevier B.V. All rights reserved. C1 [Velarde, Luis; Wang, Hong-fei] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. RP Wang, HF (reprint author), Pacific NW Natl Lab, Environm Mol Sci Lab, POB 999, Richland, WA 99352 USA. EM hongfei.wang@pnnl.gov RI Wang, Hongfei/B-1263-2010; Velarde, Luis/D-4929-2011 OI Wang, Hongfei/0000-0001-8238-1641; Velarde, Luis/0000-0001-6329-3486 FU Pacific Northwest National Laboratory (PNNL) LDRD program; Department of Energy's Office of Biological and Environmental Research (BER) FX H.F.W. thanks Ron Shen, Paulo Miranda and Steve Baldelli for valuable discussions. Paulo Miranda also suggested to measure the -CH3 group PNA of 5CT to confirm the -CN results. This work was supported by the Pacific Northwest National Laboratory (PNNL) LDRD program, and was conducted at the William R. Wiley Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility located at the Pacific Northwest National Laboratory and sponsored by the Department of Energy's Office of Biological and Environmental Research (BER). NR 33 TC 14 Z9 14 U1 4 U2 44 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2614 J9 CHEM PHYS LETT JI Chem. Phys. Lett. PD OCT 14 PY 2013 VL 585 BP 42 EP 48 DI 10.1016/j.cplett.2013.07.052 PG 7 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 228EQ UT WOS:000325169000008 ER PT J AU Pham, HH Taylor, CD Henson, NJ AF Pham, Hieu H. Taylor, Christopher D. Henson, Neil J. TI Metal desorption from Fe(110) and its alloyed surfaces SO CHEMICAL PHYSICS LETTERS LA English DT Article ID EPITAXIAL-GROWTH; SI(100) SURFACE; SI-ADATOM; CORROSION; DIFFUSION; STEEL; ELEMENTS; DISSOLUTION; TRANSITION; OXIDATION AB We have performed first-principles calculations to study the surface metal-metal bonding and energetics that control desorption on metal and alloy surfaces. The adsorbed and desorbed states of Fe, Cr, and Mo adatoms on the Fe(110) surface were examined. Their formation and extraction were investigated both as neutral particles and as metal complexes. In addition, the roles which alloying elements play on adatom-surface binding is also a critical question that needs to be addressed. The alloying effect was found to relate to the nature of charge transfer between alloying elements and host metals. (C) 2013 Elsevier B. V. All rights reserved. C1 [Pham, Hieu H.; Taylor, Christopher D.; Henson, Neil J.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Taylor, CD (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM cdtaylor@lanl.gov RI Pham, Hieu/C-6436-2015; OI Henson, Neil/0000-0002-1842-7884 FU Laboratory Directed Research and Development Early Career Program; The Los Alamos National Laboratory is operated by Los Alamos National Security LLC for the National Nuclear Security Administration of the US Department of Energy [DE-AC52-06NA25396] FX This Letter was performed at Los Alamos National Laboratory (LANL), and we gratefully acknowledge funding for this project through the Laboratory Directed Research and Development Early Career Program. The authors acknowledge the use of high performance computing resources through the Institutional Computing Program at LANL for the completion of this research. The Los Alamos National Laboratory is operated by Los Alamos National Security LLC for the National Nuclear Security Administration of the US Department of Energy under contract DE-AC52-06NA25396. NR 43 TC 1 Z9 1 U1 2 U2 20 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2614 J9 CHEM PHYS LETT JI Chem. Phys. Lett. PD OCT 14 PY 2013 VL 585 BP 162 EP 166 DI 10.1016/j.cplett.2013.09.011 PG 5 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 228EQ UT WOS:000325169000031 ER PT J AU Gu, XD Gunkel, I Russell, TP AF Gu, Xiaodan Gunkel, Ilja Russell, Thomas P. TI Pattern transfer using block copolymers SO PHILOSOPHICAL TRANSACTIONS OF THE ROYAL SOCIETY A-MATHEMATICAL PHYSICAL AND ENGINEERING SCIENCES LA English DT Review DE block copolymer; self-assembly; pattern transfer; lithography; nanotechnology ID SEQUENTIAL INFILTRATION SYNTHESIS; NANOPOROUS THIN-FILMS; SELF-ASSEMBLED NANOSTRUCTURES; MAGNETIC NANODOT ARRAYS; ABC TRIBLOCK COPOLYMERS; DIBLOCK COPOLYMER; ORDERED ARRAYS; BOTTOM-UP; TOP-DOWN; NANOLITHOGRAPHIC APPLICATIONS AB To meet the increasing demand for patterning smaller feature sizes, a lithography technique is required with the ability to pattern sub-20 nm features. While top-down photolithography is approaching its limit in the continued drive to meet Moore's law, the use of directed self-assembly (DSA) of block copolymers (BCPs) offers a promising route to meet this challenge in achieving nanometre feature sizes. Recent developments in BCP lithography and in the DSA of BCPs are reviewed. While tremendous advances have been made in this field, there are still hurdles that need to be overcome to realize the full potential of BCPs and their actual use. C1 [Gu, Xiaodan; Gunkel, Ilja; Russell, Thomas P.] Univ Massachusetts, Dept Polymer Sci & Engn, Amherst, MA 01003 USA. [Gunkel, Ilja] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Russell, TP (reprint author), Univ Massachusetts, Dept Polymer Sci & Engn, 120 Governors Dr, Amherst, MA 01003 USA. EM russell@mail.pse.umass.edu RI Gu, Xiaodan/E-9379-2015; Gu, Xiaodan/G-4029-2015; OI Gunkel, Ilja/0000-0001-5738-5309 FU US Department of Energy BES [BES-DE-FG02-96ER45612]; US Department of Energy [DE-AC02-05CH11231]; ALS FX This work was supported by the US Department of Energy BES under contract no. BES-DE-FG02-96ER45612, and by the US Department of Energy under contract no. DE-AC02-05CH11231. X. G. acknowledges the ALS Doctoral Fellowship programme for providing partial financial support. I. G. acknowledges the support of the ALS Postdoctoral Fellowship programme. NR 163 TC 23 Z9 23 U1 7 U2 95 PU ROYAL SOC PI LONDON PA 6-9 CARLTON HOUSE TERRACE, LONDON SW1Y 5AG, ENGLAND SN 1364-503X EI 1471-2962 J9 PHILOS T R SOC A JI Philos. Trans. R. Soc. A-Math. Phys. Eng. Sci. PD OCT 13 PY 2013 VL 371 IS 2000 SI SI AR UNSP 20120306 DI 10.1098/rsta.2012.0306 PG 34 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 298GE UT WOS:000330311400005 PM 24000358 ER PT J AU Muschenborn, AD Ortega, JM Szafron, JM Szafron, DJ Maitland, DJ AF Muschenborn, Andrea D. Ortega, Jason M. Szafron, Jason M. Szafron, David J. Maitland, Duncan J. TI Porous media properties of reticulated shape memory polymer foams and mock embolic coils for aneurysm treatment SO BIOMEDICAL ENGINEERING ONLINE LA English DT Article DE Permeability; Form factor; SMP; Shape memory polymer foams; Embolic coils; FHDD; Forchheimer-Hazen-Dupuit-Darcy equation; Aneurysm treatment ID INTRACRANIAL ANEURYSMS; DETACHABLE COILS; RISK-FACTORS; BLOOD-FLOW; PERMEABILITY; DYNAMICS; EMBOLIZATION; SIMULATION; STROKE; LIFE AB Background: Shape memory polymer (SMP) foams are being investigated as an alternative aneurysm treatment method to embolic coils. The goal of both techniques is the reduction of blood flow into the aneurysm and the subsequent formation of a stable thrombus, which prevents future aneurysm rupture. The purpose of this study is to experimentally determine the parameters, permeability and form factor, which are related to the flow resistance imposed by both media when subjected to a pressure gradient. Methods: The porous media properties-permeability and form factor-of SMP foams and mock embolic coils (MECs) were measured with a pressure gradient method by means of an in vitro closed flow loop. We implemented the Forchheimer-Hazen-Dupuit-Darcy equation to calculate these properties. Mechanically-reticulated SMP foams were fabricated with average cell sizes of 0.7E-3 and 1.1E-3 m, while the MECs were arranged with volumetric packing densities of 11-28%. Results: The permeability of the SMP foams was an order of magnitude lower than that of the MECs. The form factor differed by up to two orders of magnitude and was higher for the SMP foams in all cases. The maximum flow rate of all samples tested was within the inertial laminar flow regime, with Reynolds numbers ranging between 1 and 35. Conclusions: The SMP foams impose a greater resistance to fluid flow compared to MECs, which is a result of increased viscous and inertial losses. These results suggest that aneurysms treated with SMP foam will have flow conditions more favorable for blood stasis than those treated with embolic coils having packing densities <= 28%. C1 [Muschenborn, Andrea D.; Szafron, Jason M.; Szafron, David J.; Maitland, Duncan J.] Texas A&M Univ, College Stn, TX 77843 USA. [Ortega, Jason M.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RP Maitland, DJ (reprint author), Texas A&M Univ, 3120 TAMU, College Stn, TX 77843 USA. EM djmaitland@tamu.edu FU National Institutes of Health/National Institute of Biomedical Imaging and Bioengineering [R01EB000462] FX The authors thank Julie Johnson, Daniel Petty, Thomas Wilson, Pooja Singhal, Ward Small, Richard Patlan, and Matthew Tucker for their assistance in this study. This work was supported by the National Institutes of Health/National Institute of Biomedical Imaging and Bioengineering Grant R01EB000462. NR 44 TC 5 Z9 5 U1 1 U2 20 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1475-925X J9 BIOMED ENG ONLINE JI Biomed. Eng. Online PD OCT 12 PY 2013 VL 12 AR 103 DI 10.1186/1475-925X-12-103 PG 13 WC Engineering, Biomedical SC Engineering GA 247PA UT WOS:000326629500001 PM 24120254 ER PT J AU Reardon, PN Mueller, KT AF Reardon, Patrick N. Mueller, Karl T. TI Structure of the Type IVa Major Pilin from the Electrically Conductive Bacterial Nanowires of Geobacter sulfurreducens SO JOURNAL OF BIOLOGICAL CHEMISTRY LA English DT Article ID EXTRACELLULAR ELECTRON-TRANSFER; METALLIC-LIKE CONDUCTIVITY; MICROBIAL NANOWIRES; PILUS STRUCTURE; FUEL-CELLS; REDUCTION; CRYSTALLOGRAPHY; SYSTEM; RESPIRATION; SHEWANELLA AB Several species of delta proteobacteria are capable of reducing insoluble metal oxides as well as other extracellular electron acceptors. These bacteria play a critical role in the cycling of minerals in subsurface environments, sediments, and ground-water. In some species of bacteria such as Geobacter sulfurreducens, the transport of electrons is proposed to be facilitated by filamentous fibers that are referred to as bacterial nanowires. These nanowires are polymeric assemblies of proteins belonging to the type IVa family of pilin proteins and are mainly comprised of one subunit protein, PilA. Here, we report the high resolution solution NMR structure of the PilA protein from G. sulfurreducens determined in detergent micelles. The protein is > 85% alpha-helical and exhibits similar architecture to the N-terminal regions of other non-conductive type IVa pilins. The detergent micelle interacts with the first 21 amino acids of the protein, indicating that this region likely associates with the bacterial inner membrane prior to fiber formation. A model of the G. sulfurreducens pilus fiber is proposed based on docking of this structure into the fiber model of the type IVa pilin from Neisseria gonorrhoeae. This model provides insight into the organization of aromatic amino acids that are important for electrical conduction. C1 [Reardon, Patrick N.; Mueller, Karl T.] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99354 USA. [Mueller, Karl T.] Penn State Univ, Dept Chem, University Pk, PA 16802 USA. RP Reardon, PN (reprint author), Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99354 USA. EM Patrick.reardon@pnnl.gov RI Mueller, Karl/A-3637-2010; OI Reardon, Patrick/0000-0002-6858-0086 FU William Wiley Post-Doctoral Fellowship from the Environmental Molecular Sciences Laboratory; Department of Energy's Office of Biological and Environmental Research FX This work was supported by the William Wiley Post-Doctoral Fellowship from the Environmental Molecular Sciences Laboratory. All data were collected at the Environmental Molecular Sciences Laboratory, a national scientific user facility supported by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. NR 43 TC 29 Z9 31 U1 5 U2 46 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 0021-9258 EI 1083-351X J9 J BIOL CHEM JI J. Biol. Chem. PD OCT 11 PY 2013 VL 288 IS 41 BP 29260 EP 29266 DI 10.1074/jbc.M113.498527 PG 7 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA 302OT UT WOS:000330615300006 PM 23965997 ER PT J AU Wan, W Bian, W McDonald, M Kijac, A Wemmer, DE Stubbs, G AF Wan, William Bian, Wen McDonald, Michele Kijac, Aleksandra Wemmer, David E. Stubbs, Gerald TI Heterogeneous Seeding of a Prion Structure by a Generic Amyloid Form of the Fungal Prion-forming Domain HET-s(218-289) SO JOURNAL OF BIOLOGICAL CHEMISTRY LA English DT Article ID HET-S PRION; RAY FIBER DIFFRACTION; PODOSPORA-ANSERINA; PROTEIN; FIBRILS; MODEL; CORE; MICROSCOPY; AGGREGATE; MECHANISM AB The fungal prion-forming domain HET-s(218-289) forms infectious amyloid fibrils at physiological pH that were shown by solid-state NMR to be assemblies of a two-rung beta-solenoid structure. Under acidic conditions, HET-s(218-289) has been shown to form amyloid fibrils that have very low infectivity in vivo, but structural information about these fibrils has been very limited. Weshow by x-ray fiber diffraction that the HET-s(218289) fibrils formed under acidic conditions have a stacked beta-sheet architecture commonly found in short amyloidogenic peptides and denatured protein aggregates. At physiological pH, stacked beta-sheet fibrils nucleate the formation of the infectious beta-solenoid prions in a process of heterogeneous seeding, but do so with kinetic profiles distinct from those of spontaneous or homogeneous (seeded with infectious beta-solenoid fibrils) fibrillization. Several serial passages of stacked beta-sheet-seeded solutions lead to fibrillization kinetics similar to homogeneously seeded solutions. Our results directly show that structural mutation can occur between substantially different amyloid architectures, lending credence to the suggestion that the processes of strain adaptation and crossing species barriers are facilitated by structural mutation. C1 [Wan, William; Bian, Wen; McDonald, Michele; Stubbs, Gerald] Vanderbilt Univ, Dept Biol Sci, Nashville, TN 37232 USA. [Wan, William; Bian, Wen; McDonald, Michele; Stubbs, Gerald] Vanderbilt Univ, Struct Biol Ctr, Nashville, TN 37232 USA. [Kijac, Aleksandra; Wemmer, David E.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Kijac, Aleksandra; Wemmer, David E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Kijac, Aleksandra] Univ Calif San Francisco, Inst Neurodegenerat Dis, San Francisco, CA 94143 USA. RP Stubbs, G (reprint author), Vanderbilt Univ, Dept Biol Sci, 1210 MRB 3,465 21st Ave South, Nashville, TN 37232 USA. EM gerald.stubbs@vanderbilt.edu RI ID, BioCAT/D-2459-2012 FU Department of Energy; National Institutes of Health FX We thank the staff of beamline 4-2 at the Stanford Synchrotron Radiation Lightsource (SSRL) and BioCAT at the Advanced Photon Source (APS), Amy Kendall for discussions and assistance with data collection, Xi Meng for purification of the labeled HET-s protein, and Jochem Struppe of Bruker Biospin for help with pulse sequence implementation. The SSRL is a national user facility operated by Stanford University on behalf of the Department of Energy. The SSRL Structural Molecular Biology Program is supported by the Department of Energy and National Institutes of Health. The APS is supported by the Department of Energy. BioCAT and BioCARS are supported by the National Institutes of Health. NR 53 TC 9 Z9 9 U1 0 U2 11 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 0021-9258 EI 1083-351X J9 J BIOL CHEM JI J. Biol. Chem. PD OCT 11 PY 2013 VL 288 IS 41 BP 29604 EP 29612 DI 10.1074/jbc.M113.505511 PG 9 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA 302OT UT WOS:000330615300036 PM 23986444 ER PT J AU Baca, FJ Haugan, TJ Barnes, PN Holesinger, TG Maiorov, B Lu, RT Wang, X Reichart, JN Wu, JZ AF Baca, F. Javier Haugan, Timothy J. Barnes, Paul N. Holesinger, Terry G. Maiorov, Boris Lu, Rongtao Wang, Xiang Reichart, Joshua N. Wu, Judy Z. TI Interactive Growth Effects of Rare-Earth Nanoparticles on Nanorod Formation in YBa2Cu3Ox Thin Films SO ADVANCED FUNCTIONAL MATERIALS LA English DT Article DE self-assembly; BaZrO3 nanorods; thin film growth; Y2O3 nanoparticles; YBCO superconductors ID COLUMNAR DEFECTS AB The controlled growth of self-assembled second-phase nanostructures has been shown to be an essential tool for enhancing properties of several composite oxide thin film systems. Here, the role of Y2O3 nanoparticles on the growth of BaZrO3 (BZO) nanorods is investigated in order to understand the mechanisms governing their self-assembly in YBa2Cu3O7-x (YBCO) thin films and to more fully control the resulting defect landscape. By examining the microstructure and current-carrying capacity of BZO-doped YBCO films, it is shown that the nanorod growth dynamics are significantly enhanced when compared to films double-doped with BZO and Y2O3 nanoparticles. The average nanorod length and associated critical current densities are found to increase at a significantly higher rate in the absence of Y2O3 nanoparticles when the growth temperature is increased. Using microstructural data from transmission electron microscopy studies and the response in critical current density, the interactive effects of multiple dopants that must be considered to fully control the defect landscape in oxide thin films are shown. C1 [Baca, F. Javier; Holesinger, Terry G.; Maiorov, Boris] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Baca, F. Javier; Haugan, Timothy J.; Barnes, Paul N.; Reichart, Joshua N.] US Air Force Res Lab, Prop Directorate, Wright Patterson AFB, OH 45433 USA. [Baca, F. Javier; Lu, Rongtao; Wang, Xiang; Wu, Judy Z.] Univ Kansas, Dept Phys & Astron, Lawrence, KS 66045 USA. RP Baca, FJ (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM f.javier.baca@gmail.com; rtlu@ku.edu; jwu@ku.edu FU Air Force Office of Scientific Research; Department of Energy Office of Electricity; NSF [NSF-DMR-0803149, NSF-DMR-1105986, NSF EPSCoR-0903806] FX The authors acknowledge support from the Air Force Office of Scientific Research, and the Department of Energy Office of Electricity. J.Z.W. acknowledges support from NSF contracts NSF-DMR-0803149, -1105986, and NSF EPSCoR-0903806, and matching support from the State of Kansas through the Kansas Technology Enterprise Corporation. NR 36 TC 12 Z9 12 U1 5 U2 42 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1616-301X EI 1616-3028 J9 ADV FUNCT MATER JI Adv. Funct. Mater. PD OCT 11 PY 2013 VL 23 IS 38 BP 4826 EP 4831 DI 10.1002/adfm.201203660 PG 6 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 258SO UT WOS:000327479200007 ER PT J AU Liedel, C Schindler, KA Pavan, MJ Lewin, C Pester, CW Ruppel, M Urban, VS Shenhar, R Boker, A AF Liedel, Clemens Schindler, Kerstin A. Pavan, Mariela J. Lewin, Christian Pester, Christian W. Ruppel, Markus Urban, Volker S. Shenhar, Roy Boeker, Alexander TI Electric-Field-Induced Alignment of Block Copolymer/Nanoparticle Blends SO SMALL LA English DT Article DE alignment; block copolymers; electric field; nanocomposites; nanoparticles ID COPOLYMER THIN-FILMS; GOLD NANOPARTICLES; DIBLOCK COPOLYMERS; MICRODOMAIN ORIENTATION; POLYMER NANOCOMPOSITES; MICROPHASE SEPARATION; TRIBLOCK TERPOLYMERS; TRANSITION; MICROSTRUCTURE; COMPOSITES AB External electric fields readily align birefringent block-copolymer mesophases. In this study the effect of gold nanoparticles on the electric-field-induced alignment of a lamellae-forming polystyrene-block-poly(2-vinylpyridine) copolymer is assessed. Nanoparticles are homogeneously dispersed in the styrenic phase and promote the quantitative alignment of lamellar domains by substantially lowering the critical field strength above which alignment proceeds. The results suggest that the electric-field-assisted alignment of nanostructured block copolymer/nanoparticle composites may offer a simple way to greatly mitigate structural and orientational defects of such films under benign experimental conditions. C1 [Liedel, Clemens; Schindler, Kerstin A.; Lewin, Christian; Pester, Christian W.; Boeker, Alexander] Rhein Westfal TH Aachen, D-52056 Aachen, Germany. [Liedel, Clemens; Schindler, Kerstin A.; Lewin, Christian; Pester, Christian W.; Boeker, Alexander] RWTH Aachen eV, DWI, D-52056 Aachen, Germany. [Pavan, Mariela J.; Shenhar, Roy] Hebrew Univ Jerusalem, Inst Chem, IL-91904 Jerusalem, Israel. [Pavan, Mariela J.; Shenhar, Roy] Hebrew Univ Jerusalem, Ctr Nanosci & Nanotechnol, IL-91904 Jerusalem, Israel. [Ruppel, Markus] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Urban, Volker S.] Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA. RP Boker, A (reprint author), Rhein Westfal TH Aachen, Forckenbeckstr 50, D-52056 Aachen, Germany. EM boeker@dwi.rwth-aachen.de RI Boker, Alexander/C-2055-2009; Shenhar, Roy/D-8160-2011; Urban, Volker/N-5361-2015; Liedel, Clemens/A-6671-2016 OI Boker, Alexander/0000-0002-5760-6631; Shenhar, Roy/0000-0002-0631-1542; Urban, Volker/0000-0002-7962-3408; Liedel, Clemens/0000-0002-2323-9431 FU European Union; German Science Foundation (DFG) [BO 2475/5-1]; U.S. Department of Energy, Office of Science, Basic Energy Science, Materials Sciences and Engineering Division FX C. Liedel and K. A. Schindler contributed equally to this work. We thank Carmen Kunert for staining the composite films for TEM measurements and Manuel Noack and Sarah Klinkhart for help in the laboratory. Fruitful discussions with G. J. Agur Sevink, Andrei V. Zvelindovsky, Nir Tessler, and Franz Fischer are gratefully acknowledged. We thank the European Union and the German Science Foundation (DFG, BO 2475/5-1) for financial support in the framework of the ERA-NanoSci+ project MEMORY. M. R. and V.S.U. were supported by the U.S. Department of Energy, Office of Science, Basic Energy Science, Materials Sciences and Engineering Division. NR 57 TC 11 Z9 11 U1 3 U2 55 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1613-6810 EI 1613-6829 J9 SMALL JI Small PD OCT 11 PY 2013 VL 9 IS 19 BP 3276 EP 3281 DI 10.1002/smll.201202380 PG 6 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 264SD UT WOS:000327899900014 PM 23495246 ER PT J AU Salmistraro, M Schwartzberg, A Bao, W Depero, LE Weber-Bargioni, A Cabrini, S Alessandri, I AF Salmistraro, Marco Schwartzberg, Adam Bao, Wei Depero, Laura E. Weber-Bargioni, Alexander Cabrini, Stefano Alessandri, Ivano TI Triggering and Monitoring Plasmon-Enhanced Reactions by Optical Nanoantennas Coupled to Photocatalytic Beads SO SMALL LA English DT Article DE nanoantennas; nanofabrication; photocatalysis; SERS; core; shell materials ID GOLD NANOPARTICLES; VISIBLE-LIGHT; SOLAR; NANOSTRUCTURES; SPECTROSCOPY; CONVERSION; NANORODS; ENERGY; OXIDE; SIZE AB Plasmonic metal/semiconductor nanocomposites promise to be a breakthrough for boosting and investigating photon-assisted processes at the nanoscale, with exciting perspectives for energy conversion and catalysis. However, the efficiency and selectivity of these surface processes are still far from being controlled. Here, shown for the first time, is a new class of photocatalyst which is based on the synergistic combination of bowtie-like gold nanoantennas and SiO2/TiO2 core/shell oxide beads. These systems are exploited as efficient near-field optical light concentrators, stimulating photon-driven processes at the metal-semiconductor interface. Extraordinary enhancements of photodegradation rates (minutes instead of hours) result from matching the nanoantenna surface plasmon resonance with the optical absorption of organic dyes and the excitation source wavelength. Moreover, strong Raman enhancements are observed allowing for direct in-situ monitoring of reaction progress of different analytes on the same site. C1 [Salmistraro, Marco; Depero, Laura E.; Alessandri, Ivano] Univ Brescia, INSTM, I-25123 Brescia, Italy. [Salmistraro, Marco; Depero, Laura E.; Alessandri, Ivano] Univ Brescia, Chem Technol Lab, I-25123 Brescia, Italy. [Schwartzberg, Adam; Bao, Wei; Weber-Bargioni, Alexander; Cabrini, Stefano] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. RP Schwartzberg, A (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. EM amschwartzberg@lbl.gov; ivano.alessandri@ing.unibs.it RI Bao, Wei/B-4520-2014; Foundry, Molecular/G-9968-2014; Depero, Laura Eleonora/A-3176-2009 OI Depero, Laura Eleonora/0000-0001-7818-3212 FU Mechanical and Industrial Engineering Dept. of the University of Brescia; Office of Science, Office of Basic Energy Sciences, of the US Department of Energy [DE-AC02-05CH11231] FX Dr. Scott Duhey (Molecular Foundry) is acknowledged for preliminary deposition of reference planar bowtie-like nanoantennas. This work was supported by a "PID"-grant-in-aid project from the Mechanical and Industrial Engineering Dept. of the University of Brescia. Work at the Molecular Foundry was supported by the Office of Science, Office of Basic Energy Sciences, of the US Department of Energy under Contract No. DE-AC02-05CH11231. NR 35 TC 27 Z9 27 U1 14 U2 130 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1613-6810 EI 1613-6829 J9 SMALL JI Small PD OCT 11 PY 2013 VL 9 IS 19 BP 3301 EP 3307 DI 10.1002/smll.201300211 PG 7 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 264SD UT WOS:000327899900017 PM 23606587 ER PT J AU Zhu, YJ Wang, JW Liu, Y Liu, XH Kushima, A Liu, YH Xu, YH Mao, SX Li, J Wang, CS Huang, JY AF Zhu, Yujie Wang, Jiang Wei Liu, Yang Liu, Xiaohua Kushima, Akihiro Liu, Yihang Xu, Yunhua Mao, Scott X. Li, Ju Wang, Chunsheng Huang, Jian Yu TI In Situ Atomic-Scale Imaging of Phase Boundary Migration in FePO4 Microparticles During Electrochemical Lithiation SO ADVANCED MATERIALS LA English DT Article DE LiFePO4; Lithium; batteries; in situ TEM; imaging; microparticles ID LIFEPO4 NANOPARTICLES; LI-INSERTION/EXTRACTION; BATTERY MATERIALS; TRANSITION; ELECTRODES; DELITHIATION; SEPARATION; NANOWIRES; DISCHARGE; PATHWAYS C1 [Zhu, Yujie; Liu, Yang; Xu, Yunhua; Wang, Chunsheng] Univ Maryland, Dept Chem & Biomol Engn, College Pk, MD 20742 USA. [Wang, Jiang Wei; Mao, Scott X.] Univ Pittsburgh, Dept Mech Engn & Mat Sci, Pittsburgh, PA 15261 USA. [Liu, Yang; Liu, Xiaohua; Huang, Jian Yu] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA. [Kushima, Akihiro; Li, Ju] MIT, Dept Nucl Sci & Engn, Cambridge, MA 02139 USA. [Kushima, Akihiro; Li, Ju] MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA. RP Li, J (reprint author), MIT, Dept Nucl Sci & Engn, 77 Massachusetts Ave, Cambridge, MA 02139 USA. EM liju@mit.edu; cswang@umd.edu; jyhuang8@yahoo.com RI Li, Ju/A-2993-2008; Wang, Jiangwei/F-8249-2011; Wang, Chunsheng/H-5767-2011; Liu, Xiaohua/A-8752-2011; Liu, Yihang/E-6958-2013; Kushima, Akihiro/H-2347-2011 OI Li, Ju/0000-0002-7841-8058; Wang, Jiangwei/0000-0003-1191-0782; Wang, Chunsheng/0000-0002-8626-6381; Liu, Xiaohua/0000-0002-7300-7145; Liu, Yihang/0000-0002-2491-9439; FU Nanostructures for Electrical Energy Storage, an Energy Frontier Research Center; U.S. Department of Energy, Office of Science; Office of Basic Energy Sciences [DESC0001160]; National Science Foundation [CBET0933228]; NSF [DMR-1008104, DMR-1120901]; Laboratory Directed Research and Development (LDRD) project at Sandia National Laboratories (SNL); U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work is supported as part of the Nanostructures for Electrical Energy Storage, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, and Office of Basic Energy Sciences under Award Number DESC0001160. Financial support in part by the National Science Foundation under Contract No. CBET0933228 (Dr. Maria Burka, Program Director) is gratefully acknowledged. A. K. and J. L. acknowledge support by NSF DMR-1008104 and DMR-1120901. The authors acknowledge the technical support of the NanoCenter in University of Maryland. Portions of this work were supported by a Laboratory Directed Research and Development (LDRD) project at Sandia National Laboratories (SNL). The LDRD supported the development and fabrication of platforms. The NEES center supported the development of TEM techniques. CINT supported the TEM capability. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 35 TC 38 Z9 38 U1 15 U2 134 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD OCT 11 PY 2013 VL 25 IS 38 BP 5461 EP 5466 DI 10.1002/adma.201301374 PG 6 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 262RY UT WOS:000327756500006 PM 23873760 ER PT J AU Griffith, OL Pepin, F Enache, OM Heiser, LM Collisson, EA Spellman, PT Gray, JW AF Griffith, Obi L. Pepin, Francois Enache, Oana M. Heiser, Laura M. Collisson, Eric A. Spellman, Paul T. Gray, Joe W. TI A robust prognostic signature for hormone-positive node-negative breast cancer SO GENOME MEDICINE LA English DT Article ID EXPRESSION SIGNATURE; HISTOLOGIC GRADE; GENECHIP DATA; THERAPY; SURVIVAL; RECURRENCE; SUBTYPES AB Background: Systemic chemotherapy in the adjuvant setting can cure breast cancer in some patients that would otherwise recur with incurable, metastatic disease. However, since only a fraction of patients would have recurrence after surgery alone, the challenge is to stratify high-risk patients (who stand to benefit from systemic chemotherapy) from low-risk patients (who can safely be spared treatment related toxicities and costs). Methods: We focus here on risk stratification in node-negative, ER-positive, HER2-negative breast cancer. We use a large database of publicly available microarray datasets to build a random forests classifier and develop a robust multi-gene mRNA transcription-based predictor of relapse free survival at 10 years, which we call the Random Forests Relapse Score (RFRS). Performance was assessed by internal cross-validation, multiple independent data sets, and comparison to existing algorithms using receiver-operating characteristic and Kaplan-Meier survival analysis. Internal redundancy of features was determined using k-means clustering to define optimal signatures with smaller numbers of primary genes, each with multiple alternates. Results: Internal OOB cross-validation for the initial (full-gene-set) model on training data reported an ROC AUC of 0.704, which was comparable to or better than those reported previously or obtained by applying existing methods to our dataset. Three risk groups with probability cutoffs for low, intermediate, and high-risk were defined. Survival analysis determined a highly significant difference in relapse rate between these risk groups. Validation of the models against independent test datasets showed highly similar results. Smaller 17-gene and 8-gene optimized models were also developed with minimal reduction in performance. Furthermore, the signature was shown to be almost equally effective on both hormone-treated and untreated patients. Conclusions: RFRS allows flexibility in both the number and identity of genes utilized from thousands to as few as 17 or eight genes, each with multiple alternatives. The RFRS reports a probability score strongly correlated with risk of relapse. This score could therefore be used to assign systemic chemotherapy specifically to those high-risk patients most likely to benefit from further treatment. C1 [Griffith, Obi L.; Pepin, Francois; Enache, Oana M.; Heiser, Laura M.; Spellman, Paul T.; Gray, Joe W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Dept Canc & DNA Damage Responses, Berkeley, CA 94720 USA. [Heiser, Laura M.; Gray, Joe W.] Oregon Hlth & Sci Univ, Knight Canc Inst, Ctr Spatial Syst Biomed, Dept Biomed Engn, Portland, OR USA. [Collisson, Eric A.] Univ Calif San Francisco, Div Hematol Oncol, San Francisco, CA 94143 USA. RP Griffith, OL (reprint author), Washington Univ, Dept Med, Div Oncol, Genome Inst, Campus Box 8501,4444 Forest Pk Ave, St Louis, MO 63108 USA. EM obigriffith@wustl.edu; spellmap@ohsu.edu; grayjo@ohsu.edu OI Griffith, Obi/0000-0002-0843-4271 FU Canadian Institutes of Health Research. EAC [K08 CA137153]; NCI ICBP Summer Cancer Research Fellowship program; Director, Office of Science, Office of Biological & Environmental Research; U.S. Department of Energy [DE-AC02-05CH11231, U54 CA 112970]; [SU2C-AACR-DT0409] FX OLG was supported by a Fellowship from the Canadian Institutes of Health Research. EAC was supported by K08 CA137153. OME was supported by the NCI ICBP Summer Cancer Research Fellowship program. This work was supported by the Director, Office of Science, Office of Biological & Environmental Research, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231; U54 CA 112970 and SU2C-AACR-DT0409 to JWG. The content of the information does not necessarily reflect the position or the policy of the Government, and no official endorsement should be NR 29 TC 7 Z9 7 U1 0 U2 3 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1756-994X J9 GENOME MED JI Genome Med. PD OCT 11 PY 2013 VL 5 AR 92 DI 10.1186/gm496 PG 14 WC Genetics & Heredity SC Genetics & Heredity GA 246OY UT WOS:000326549600002 PM 24112773 ER PT J AU Chen, JF Marks, E Lai, B Zhang, ZJ Duce, JA Lam, LQ Volitakis, I Bush, AI Hersch, S Fox, JH AF Chen, Jianfang Marks, Eileen Lai, Barry Zhang, Zhaojie Duce, James A. Lam, Linh Q. Volitakis, Irene Bush, Ashley I. Hersch, Steven Fox, Jonathan H. TI Iron Accumulates in Huntington's Disease Neurons: Protection by Deferoxamine SO PLOS ONE LA English DT Article ID AMYLOID PRECURSOR PROTEIN; MOUSE MODEL; PARKINSONS-DISEASE; OXIDATIVE STRESS; NEURODEGENERATIVE DISEASES; MITOCHONDRIAL DYSFUNCTION; ALZHEIMERS-DISEASE; TRANSGENIC MOUSE; BASAL GANGLIA; HD MUTATION AB Huntington's disease (HD) is a progressive neurodegenerative disorder caused by a polyglutamine-encoding CAG expansion in the huntingtin gene. Iron accumulates in the brains of HD patients and mouse disease models. However, the cellular and subcellular sites of iron accumulation, as well as significance to disease progression are not well understood. We used independent approaches to investigate the location of brain iron accumulation. In R6/2 HD mouse brain, synchotron x-ray fluorescence analysis revealed iron accumulation as discrete puncta in the perinuclear cytoplasm of striatal neurons. Further, perfusion Turnbull's staining for ferrous iron (II) combined with transmission electron microscope ultra-structural analysis revealed increased staining in membrane bound perinuclear vesicles in R6/2 HD striatal neurons. Analysis of iron homeostatic proteins in R6/2 HD mice revealed decreased levels of the iron response proteins (IRPs 1 and 2) and accordingly decreased expression of iron uptake transferrin receptor (TfR) and increased levels of neuronal iron export protein ferroportin (FPN). Finally, we show that intra-ventricular delivery of the iron chelator deferoxamine results in an improvement of the motor phenotype in R6/2 HD mice. Our data supports accumulation of redox-active ferrous iron in the endocytic / lysosomal compartment in mouse HD neurons. Expression changes of IRPs, TfR and FPN are consistent with a compensatory response to an increased intra-neuronal labile iron pool leading to increased susceptibility to iron-associated oxidative stress. These findings, together with protection by deferoxamine, support a potentiating role of neuronal iron accumulation in HD. C1 [Chen, Jianfang; Marks, Eileen; Fox, Jonathan H.] Univ Wyoming, Dept Vet Sci, Laramie, WY 82071 USA. [Chen, Jianfang; Marks, Eileen; Fox, Jonathan H.] Univ Wyoming, Grad Program Neurosci, Laramie, WY 82071 USA. [Lai, Barry] Argonne Natl Lab, Lemont, IL USA. [Zhang, Zhaojie] Univ Wyoming, Dept Zool & Physiol, Laramie, WY 82071 USA. [Duce, James A.; Lam, Linh Q.; Volitakis, Irene; Bush, Ashley I.] Mental Hlth Res Inst, Melbourne, Vic, Australia. [Duce, James A.] Univ Leeds, Fac Biol Sci, Sch Mol & Cellular Biol, Leeds, W Yorkshire, England. [Hersch, Steven] MassGen Inst Neurodegenerat Dis, Charlestown, MA USA. RP Fox, JH (reprint author), Univ Wyoming, Dept Vet Sci, Laramie, WY 82071 USA. EM jfox7@uwyo.edu RI Bush, Ashley/A-1186-2007; OI Bush, Ashley/0000-0001-8259-9069; Volitakis, Irene/0000-0003-0766-817X; Duce, James/0000-0002-8762-2245 FU National Institutes of Health; Huntington's Disease Society of America; National Center for Research Resources from the National Institutes of Health [5P30RR032128-02]; National Institute of General Medical Sciences from the National Institutes of Health [8 P30GM103398-02]; National Institute of Neurological Disorders and Stroke from the National Institutes of Health [RO1NS079450]; U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work was supported by grants from the National Institutes of Health and by the Huntington's Disease Society of America, the National Center for Research Resources (5P30RR032128-02), the National Institute of General Medical Sciences (8 P30GM103398-02) and National Institute of Neurological Disorders and Stroke (RO1NS079450) from the National Institutes of Health. Use of the Advanced Photon Source at Argonne National Laboratory was supported by the U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 59 TC 23 Z9 23 U1 2 U2 16 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD OCT 11 PY 2013 VL 8 IS 10 AR e77023 DI 10.1371/journal.pone.0077023 PG 12 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 236SL UT WOS:000325819400095 PM 24146952 ER PT J AU Li, TW Zhang, YM AF Li, Tingwen Zhang, Yongmin TI A new model for two-dimensional numerical simulation of pseudo-2D gas-solids fluidized beds SO CHEMICAL ENGINEERING SCIENCE LA English DT Article DE Computational fluid dynamics; Fluidized bed; Pseudo-2D system; Gas-solids flow; Two-fluid model; Wall friction ID DIGITAL IMAGE-ANALYSIS; BOUNDARY-CONDITIONS; GRANULAR-MATERIALS; PART I; FLOW; HYDRODYNAMICS; THICKNESS; BEHAVIOR; BUBBLES; FLAT AB Pseudo two dimensional (pseudo 2D) fluidized beds, for which the thickness of the system is much smaller than the other two dimensions, are widely used to perform fundamental studies on bubble behavior, solids mixing, or clustering phenomenon in different gas solids fluidization systems. The abundant data from such experimental systems are very useful for numerical model development and validation. However, it has been reported that two-dimensional (2D) computational fluid dynamic (CFD) simulations of pseudo 2D gas solids fluidized beds usually predict poor quantitative agreement with the experimental data, especially for the solids velocity field. In this paper, a new model is proposed to improve the 2D numerical simulations of pseudo 2D gas solids fluidized beds by properly accounting for the frictional effect of the front and back walls. Two previously reported pseudo 2D experimental systems were simulated with this model. Compared to the traditional 2D simulations, significant improvements in the numerical predictions have been observed and the predicted results arc in better agreement with the available experimental data. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Li, Tingwen] Natl Energy Technol Lab, Dept Energy, Morgantown, WV 26505 USA. [Li, Tingwen] URS Corp, Morgantown, WV 26505 USA. [Zhang, Yongmin] China Univ Petr, State Key Lab Heavy Oil Proc, Beijing 102249, Peoples R China. RP Li, TW (reprint author), Natl Energy Technol Lab, Dept Energy, Morgantown, WV 26505 USA. EM tingwen.li@contr.netl.doe.gov FU RES [DE-FE0004000]; National Natural Science Foundation of China [21276273]; Ministry of Science and Technology of China [2012BAE05B02, 2012CB215004] FX This technical report was produced in support of the National Energy Technology Laboratory's ongoing research in advanced numerical simulation of multiphase flow under the RES contract DE-FE0004000. The authors also acknowledge the financial supports by the National Natural Science Foundation of China (21276273), the Ministry of Science and Technology of China (2012BAE05B02 and 2012CB215004). NR 47 TC 8 Z9 8 U1 3 U2 33 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0009-2509 EI 1873-4405 J9 CHEM ENG SCI JI Chem. Eng. Sci. PD OCT 11 PY 2013 VL 102 BP 246 EP 256 DI 10.1016/j.ces.2013.08.019 PG 11 WC Engineering, Chemical SC Engineering GA 238KP UT WOS:000325945500023 ER PT J AU Barfuss, A Dudy, L Scholz, MR Roth, H Hopfner, P Blumenstein, C Landolt, G Dil, JH Plumb, NC Radovic, M Bostwick, A Rotenberg, E Fleszar, A Bihlmayer, G Wortmann, D Li, G Hanke, W Claessen, R Schafer, J AF Barfuss, A. Dudy, L. Scholz, M. R. Roth, H. Hoepfner, P. Blumenstein, C. Landolt, G. Dil, J. H. Plumb, N. C. Radovic, M. Bostwick, A. Rotenberg, E. Fleszar, A. Bihlmayer, G. Wortmann, D. Li, G. Hanke, W. Claessen, R. Schaefer, J. TI Elemental Topological Insulator with Tunable Fermi Level: Strained alpha-Sn on InSb(001) SO PHYSICAL REVIEW LETTERS LA English DT Article ID HGTE QUANTUM-WELLS; SINGLE DIRAC CONE; RESOLVED PHOTOEMISSION; HETEROEPITAXIAL FILMS; PSEUDOMORPHIC GROWTH; ELECTRONIC-STRUCTURE; BAND STRUCTURE; SURFACE; BI2TE3; INSB AB We report on the epitaxial fabrication and electronic properties of a topological phase in strained alpha-Sn on InSb. The topological surface state forms in the presence of an unusual band order not based on direct spin-orbit coupling, as shown in density functional and GW slab-layer calculations. Angle-resolved photoemission including spin detection probes experimentally how the topological spin-polarized state emerges from the second bulk valence band. Moreover, we demonstrate the precise control of the Fermi level by dopants. C1 [Barfuss, A.; Dudy, L.; Scholz, M. R.; Roth, H.; Hoepfner, P.; Blumenstein, C.; Claessen, R.; Schaefer, J.] Univ Wurzburg, Inst Phys, D-97074 Wurzburg, Germany. [Barfuss, A.; Dudy, L.; Scholz, M. R.; Roth, H.; Hoepfner, P.; Blumenstein, C.; Claessen, R.; Schaefer, J.] Univ Wurzburg, Rontgen Ctr Complex Mat Syst, D-97074 Wurzburg, Germany. [Landolt, G.; Dil, J. H.; Plumb, N. C.; Radovic, M.] Paul Scherrer Inst, Swiss Light Source, CH-5232 Villigen, Switzerland. [Landolt, G.; Dil, J. H.] Univ Zurich, Inst Phys, CH-8057 Zurich, Switzerland. [Bostwick, A.; Rotenberg, E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Fleszar, A.; Li, G.; Hanke, W.] Univ Wurzburg, Inst Theoret Phys & Astron, D-97074 Wurzburg, Germany. [Bihlmayer, G.; Wortmann, D.] Forschungszentrum Julich, Peter Grunberg Inst, D-52425 Julich, Germany. [Bihlmayer, G.; Wortmann, D.] Forschungszentrum Julich, Inst Adv Simulat, D-52425 Julich, Germany. RP Barfuss, A (reprint author), Univ Wurzburg, Inst Phys, D-97074 Wurzburg, Germany. EM Joerg.Schaefer@physik.uni-wuerzburg.de RI Dil, Hugo/F-6995-2012; Li, Gang/E-5004-2013; Claessen, Ralph/A-2045-2017; Plumb, Nicholas/B-8059-2013; Bihlmayer, Gustav/G-5279-2013; Rotenberg, Eli/B-3700-2009 OI Dil, Hugo/0000-0002-6016-6120; Li, Gang/0000-0002-0952-5909; Claessen, Ralph/0000-0003-3682-6325; Wortmann, Daniel/0000-0002-2248-1904; Plumb, Nicholas/0000-0002-2334-8494; Bihlmayer, Gustav/0000-0002-6615-1122; Rotenberg, Eli/0000-0002-3979-8844 FU Deutsche Forschungsgemeinschaft [FOR 1162, SCHA 1510/5-1] FX We are grateful for discussion with Oliver Rader and Laurens Molenkamp. This work was supported by the Deutsche Forschungsgemeinschaft under Grants No. FOR 1162 and No. SCHA 1510/5-1. NR 33 TC 34 Z9 35 U1 5 U2 76 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 11 PY 2013 VL 111 IS 15 AR 157205 DI 10.1103/PhysRevLett.111.157205 PG 5 WC Physics, Multidisciplinary SC Physics GA 239UQ UT WOS:000326051600007 PM 24160626 ER PT J AU Hohensee, MA Muller, H Wiringa, RB AF Hohensee, Michael A. Mueller, Holger Wiringa, R. B. TI Equivalence Principle and Bound Kinetic Energy SO PHYSICAL REVIEW LETTERS LA English DT Article ID TESTS; GRAVIMETERS; GRAVITY AB We consider the role of the internal kinetic energy of bound systems of matter in tests of the Einstein equivalence principle. Using the gravitational sector of the standard model extension, we show that stringent limits on equivalence principle violations in antimatter can be indirectly obtained from tests using bound systems of normal matter. We estimate the bound kinetic energy of nucleons in a range of light atomic species using Green's function Monte Carlo calculations, and for heavier species using a Woods-Saxon model. We survey the sensitivities of existing and planned experimental tests of the equivalence principle, and report new constraints at the level of between a few parts in 10(6) and parts in 10(8) on violations of the equivalence principle for matter and antimatter. C1 [Hohensee, Michael A.; Mueller, Holger] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Wiringa, R. B.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. RP Hohensee, MA (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM hohensee@berkeley.edu RI Mueller, Holger/E-3194-2015; Wiringa, Robert/M-4970-2015; OI Hohensee, Michael/0000-0002-8106-4502 FU National Aeronautics and Space Administration [JPL-1465360]; David and Lucile Packard Foundation; U.S. Department of Energy, Office of Nuclear Physics [DE-AC02-06CH11357] FX We thank Brian Estey, Paul Hamilton, Alan Kostelecky, Anna Nobili, and Jay Tasson for stimulating discussions. M. A. H. and H. M. were supported in this work by a grant from the National Aeronautics and Space Administration (JPL-1465360), and the David and Lucile Packard Foundation. The work of R. B. W. is supported by the U.S. Department of Energy, Office of Nuclear Physics, under Contract No. DE-AC02-06CH11357. We also thank W. Nazarewicz and N. Birge for providing us with independent estimates of the bound kinetic energy of nucleons in a range of atomic species. NR 43 TC 24 Z9 24 U1 0 U2 18 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 11 PY 2013 VL 111 IS 15 AR 151102 DI 10.1103/PhysRevLett.111.151102 PG 5 WC Physics, Multidisciplinary SC Physics GA 239UQ UT WOS:000326051600002 PM 24160587 ER PT J AU Antonelli, M Cirigliano, V Lusiani, A Passemar, E AF Antonelli, Mario Cirigliano, Vincenzo Lusiani, Alberto Passemar, Emilie TI Predicting the tau strange branching ratios and implications for V-us SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Quark Masses and SM Parameters; Kaon Physics; QCD; Chiral Lagrangians ID VECTOR FORM-FACTOR; RADIATIVE-CORRECTIONS; STANDARD MODEL; KL3 DECAYS; ANALYTICITY; CONSTRAINTS; UNITARITY; SCALAR; WIDTH AB Hadronic tau decays provide several ways to extract the Cabbibo-Kobashi-Maskawa (CKM) matrix element V-us. The most precise determination involves using inclusive tau decays and requires as input the total branching ratio into strange final states. Recent results from B-factories have led to a discrepancy of about 3.4 sigma from the value of V-us implied by CKM unitarity and direct determination from Kaon semi-leptonic modes. In this paper we predict the three leading strange tau branching ratios, using dispersive parameterizations of the hadronic form factors and taking as experimental input the measured Kaon decay rates and the tau -> K pi nu(tau) decay spectrum. We then use our results to reevaluate V-us, for which we find vertical bar V-us vertical bar = 0.2207 +/- 0.0027, in better agreement with CKM unitarity. C1 [Antonelli, Mario] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Cirigliano, Vincenzo; Passemar, Emilie] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Lusiani, Alberto] Scuola Normale Super Pisa, Ist Nazl Fis Nucl, Sez Pisa, I-56127 Pisa, Italy. RP Antonelli, M (reprint author), Ist Nazl Fis Nucl, Lab Nazl Frascati, Via E Fermi 40, I-00044 Frascati, Italy. EM mario.antonelli@lnf.infn.it; cirigliano@lanl.gov; alberto.lusiani@pi.infn.it; passemar@lanl.gov RI Lusiani, Alberto/N-2976-2015; Lusiani, Alberto/A-3329-2016 OI Lusiani, Alberto/0000-0002-6876-3288; Lusiani, Alberto/0000-0002-6876-3288 FU DOE Office of Nuclear Physics; LDRD program at Los Alamos National Laboratory FX We are grateful to V. Bernard and D. R. Boito for important discussions and sharing with us unpublished results. VC and EP acknowledge support from DOE Office of Nuclear Physics and the LDRD program at Los Alamos National Laboratory. NR 38 TC 4 Z9 4 U1 0 U2 1 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD OCT 11 PY 2013 IS 10 AR 070 DI 10.1007/JHEP10(2013)070 PG 19 WC Physics, Particles & Fields SC Physics GA 233JZ UT WOS:000325565900002 ER PT J AU Rissanen, J Clark, RM Gregorich, KE Gates, JM Campbell, CM Crawford, HL Cromaz, M Esker, NE Fallon, P Forsberg, U Gothe, O Lee, IY Liu, HL Machiavelli, AO Mudder, P Nitsche, H Pang, G Rice, A Rudolph, D Stoyer, MA Wiens, A Xu, FR AF Rissanen, J. Clark, R. M. Gregorich, K. E. Gates, J. M. Campbell, C. M. Crawford, H. L. Cromaz, M. Esker, N. E. Fallon, P. Forsberg, U. Gothe, O. Lee, I. -Y. Liu, H. L. Machiavelli, A. O. Mudder, P. Nitsche, H. Pang, G. Rice, A. Rudolph, D. Stoyer, M. A. Wiens, A. Xu, F. R. TI Decay of the high-K isomeric state to a rotational band in (257)Rf SO PHYSICAL REVIEW C LA English DT Article ID MULTI-QUASI-PARTICLE; SUPERHEAVY ELEMENTS; HEAVY-ELEMENTS; NO-254; GAMMA; TRANSITIONS; FISSION; NUCLEI; REGION AB The (257)Rf isotope has been populated via the Pb-208(Ti-50, n) fusion-evaporation reaction and delayed gamma-ray and electron decay spectroscopy has been performed. The existence of a high-K isomeric state in (257)Rf has been confirmed. The isomeric state decays into a rotational band based on the 11/2(-)[725] excitation, which was observed up to spin of (23/2(-)). Three multipolarity-E1 gamma transitions depopulating the isomeric state have been observed, which fixes the spin for that state to (21/2(+)). This assignment agrees with theoretical predictions calculated with the microscopic-macroscopic approach, which suggest the isomeric state to be formed by coupling an unpaired 11/2(-)[725] quasineutron to the (1/2(-)[521] circle times 9/2(+)[624])(5)- two-quasiproton state. The same two-quasiproton excitation is possible for the lowest isomer in (256)Rf. C1 [Rissanen, J.; Clark, R. M.; Gregorich, K. E.; Gates, J. M.; Campbell, C. M.; Crawford, H. L.; Cromaz, M.; Esker, N. E.; Fallon, P.; Gothe, O.; Lee, I. -Y.; Machiavelli, A. O.; Mudder, P.; Nitsche, H.; Pang, G.; Rice, A.; Wiens, A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Esker, N. E.; Gothe, O.; Mudder, P.; Nitsche, H.; Rice, A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Forsberg, U.; Rudolph, D.] Lund Univ, SE-22100 Lund, Sweden. [Liu, H. L.] Xi An Jiao Tong Univ, Dept Appl Phys, Xian 710049, Peoples R China. [Stoyer, M. A.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Xu, F. R.] Peking Univ, Sch Phys, Beijing 100871, Peoples R China. RP Rissanen, J (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. EM juhorissanen@lbl.gov RI Rudolph, Dirk/D-4259-2009; Xu, Furong/K-4178-2013 OI Rudolph, Dirk/0000-0003-1199-3055; FU U.S. Department of Energy [DE-AC02-05CH11231, DE-AC52-07NA27344]; Swedish Research Council (LU); Royal Physiographic Society in Lund FX We are grateful to Jerome Rubert and Benoit Gall of IPHC Strasbourg for sharing with us their results on 256Rf prior to publication and for many illuminating discussions. We thank the 88-Inch Cyclotron operations staff for providing the beams for this experiment. This work was supported in part by the U.S. Department of Energy under Contract No. DE-AC02-05CH11231 (LBNL) and No. DE-AC52-07NA27344 (LLNL), and the Swedish Research Council (LU). U.F. acknowledges support from the Royal Physiographic Society in Lund. NR 47 TC 10 Z9 10 U1 1 U2 18 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD OCT 11 PY 2013 VL 88 IS 4 AR 044313 DI 10.1103/PhysRevC.88.044313 PG 9 WC Physics, Nuclear SC Physics GA 233PJ UT WOS:000325581000003 ER PT J AU Alberca, A Nemes, NM Mompean, FJ Feher, T Simon, F Tornos, J Leon, C Munuera, C Kirby, BJ Fitzsimmons, MR Hernando, A Santamaria, J Garcia-Hernandez, M AF Alberca, A. Nemes, N. M. Mompean, F. J. Feher, T. Simon, F. Tornos, J. Leon, C. Munuera, C. Kirby, B. J. Fitzsimmons, M. R. Hernando, A. Santamaria, J. Garcia-Hernandez, M. TI Magnetoelastic coupling in La0.7Ca0.3MnO3/BaTiO3 ultrathin films SO PHYSICAL REVIEW B LA English DT Article ID MAGNETIC-ANISOTROPY; OXIDES AB The magnetism of La0.7Ca0.3MnO3 (LCMO) epitaxial thin films grown on SrTiO3 (STO) and BaTiO3 (BTO) substrates is studied using polarized neutron reflectometry (PNR) and ferromagnetic resonance (FMR) techniques. In LCMO/BTO, PNR reveals a strongly suppressed magnetization of 300 kA/m, equivalent to a magnetic moment of 2 mu B/Mn, throughout the LCMO layer, amounting to half the expected value. The largest suppression occurs near the interface with BTO, with magnetization values of 50 kA/m, equivalent to 0.3 mu B/Mn. FMR is observable at 8.9 GHz only around the [110] crystallographic direction in thin LCMO/BTO. The resonance barely shifts as the applied field is rotated away from [110]. The FMR results are analyzed in terms of magnetoelastic anisotropy and compared to LCMO/STO grown under the same conditions. A two-layer magnetization model is proposed, based on strong out-of-plane anisotropy near the BTO interface and shown to qualitatively explain the main characteristics of the FMR results. C1 [Alberca, A.; Mompean, F. J.; Munuera, C.; Garcia-Hernandez, M.] CSIC, Inst Ciencia Mat Madrid, ES-28049 Madrid, Spain. [Nemes, N. M.; Tornos, J.; Leon, C.; Santamaria, J.] Univ Complutense, Dept Fis Aplicada 3, ES-28040 Madrid, Spain. [Hernando, A.] Univ Complutense, Dept Fis Mat, ES-28040 Madrid, Spain. [Hernando, A.] Univ Complutense, Inst Magnetismo Aplicado Salvador Velayos, ES-28040 Madrid, Spain. [Feher, T.; Simon, F.] Budapest Univ Technol & Econ, Dept Phys, H-1111 Budapest, Hungary. [Feher, T.; Simon, F.] Hungarian Acad Sci, Condensed Matter Res Grp, H-1111 Budapest, Hungary. [Alberca, A.; Nemes, N. M.; Mompean, F. J.; Tornos, J.; Leon, C.; Munuera, C.; Santamaria, J.; Garcia-Hernandez, M.] Univ Complutense Madrid, Unidad Asociada Consejo Super Invest Cient, Lab Heteroestruct Aplicac Spintron, ES-28049 Madrid, Spain. [Kirby, B. J.] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Fitzsimmons, M. R.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Alberca, A (reprint author), CSIC, Inst Ciencia Mat Madrid, Sor Juana Ines Cruz 3, ES-28049 Madrid, Spain. RI Leon, Carlos/A-5587-2008; Simon, Ferenc/G-7580-2011; Garcia-Hernandez, Mar/J-9520-2014; Munuera, Carmen/J-9928-2014; Mompean, Federico/B-8713-2011; Santamaria, Jacobo/N-8783-2016; Hernando, Antonio/E-2105-2015 OI Leon, Carlos/0000-0002-3262-1843; Simon, Ferenc/0000-0001-9822-4309; Garcia-Hernandez, Mar/0000-0002-5987-0647; Santamaria, Jacobo/0000-0003-4594-2686; FU Spanish Ministry for Science and Innovation [MAT2011-27470-C02-01, MAT2011-27470-C02-02, CSD2009-00013]; European Research Council [ERC-259374-Sylo]; Office of Basic Energy Science (BES), U.S. Department of Energy (DOE), BES-Department of Materials Science; DOE's Office of BES, Division of Materials Research [DE FG03-87ER-45332]; Hungarian OTKA [K107228, CNK80991]; Los Alamos National Security LLC under DOE [DE-AC52-06NA25396] FX We thank Maria Jose Calderon for useful discussions. We acknowledge funding from the Spanish Ministry for Science and Innovation through Grants No. MAT2011-27470-C02-01, No. MAT2011-27470-C02-02, and No. CSD2009-00013. Work supported by the European Research Council Starting Grant No. ERC-259374-Sylo and by the Office of Basic Energy Science (BES), U.S. Department of Energy (DOE), BES-Department of Materials Science funded by the DOE's Office of BES, Division of Materials Research under Grant No. DE FG03-87ER-45332 and Hungarian OTKA Grants K107228 and CNK80991. Los Alamos National Laboratory is operated by Los Alamos National Security LLC under DOE Contract No. DE-AC52-06NA25396. NR 49 TC 3 Z9 3 U1 4 U2 74 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 11 PY 2013 VL 88 IS 13 AR 134410 DI 10.1103/PhysRevB.88.134410 PG 12 WC Physics, Condensed Matter SC Physics GA 233GF UT WOS:000325555100001 ER PT J AU Couet, S Peelaers, H Trekels, M Houben, K Petermann, C Hu, MY Zhao, JY Bi, W Alp, EE Menendez, E Partoens, B Peeters, FM Van Bael, MJ Vantomme, A Temst, K AF Couet, S. Peelaers, H. Trekels, M. Houben, K. Petermann, C. Hu, M. Y. Zhao, J. Y. Bi, W. Alp, E. E. Menendez, E. Partoens, B. Peeters, F. M. Van Bael, M. J. Vantomme, A. Temst, K. TI Interplay between lattice dynamics and superconductivity in Nb3Sn thin films (vol 88, 045437, 2013) SO PHYSICAL REVIEW B LA English DT Correction C1 [Couet, S.; Trekels, M.; Petermann, C.; Menendez, E.; Vantomme, A.; Temst, K.] Katholieke Univ Leuven, Inst Kern & Stralingsfys, B-3001 Louvain, Belgium. [Peelaers, H.] Univ Calif Santa Barbara, Dept Mat, Santa Barbara, CA 93106 USA. [Peelaers, H.; Partoens, B.; Peeters, F. M.] Univ Antwerp, Dept Fys, B-2020 Antwerp, Belgium. [Houben, K.; Van Bael, M. J.] Katholieke Univ Leuven, Lab Vaste Stoffys & Magnetisme, B-3001 Louvain, Belgium. [Hu, M. Y.; Zhao, J. Y.; Bi, W.; Alp, E. E.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Bi, W.] Univ Illinois, Dept Geol, Urbana, IL 61801 USA. RP Couet, S (reprint author), Katholieke Univ Leuven, Inst Kern & Stralingsfys, Celestijnenlaan 200D, B-3001 Louvain, Belgium. RI Van Bael, Margriet/D-5382-2015; CMT, UAntwerpen Group/A-5523-2016; Menendez, Enric /E-2469-2016 OI Menendez, Enric /0000-0003-3809-2863 NR 1 TC 0 Z9 0 U1 2 U2 15 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 11 PY 2013 VL 88 IS 15 AR 159903 DI 10.1103/PhysRevB.88.159903 PG 1 WC Physics, Condensed Matter SC Physics GA 233IK UT WOS:000325561500006 ER PT J AU Dong, S Dagotto, E AF Dong, Shuai Dagotto, Elbio TI Full control of magnetism in a manganite bilayer by ferroelectric polarization SO PHYSICAL REVIEW B LA English DT Article ID TUNNEL-JUNCTIONS; SPIN POLARIZATION; ROOM-TEMPERATURE; ELECTRIC CONTROL; EXCHANGE BIAS; THIN-FILMS; INTERFACES; FERROMAGNETISM; LAYERS AB An oxide heterostructure made of manganite bilayers and ferroelectric perovskites is predicted to lead to the full control of magnetism when switching the ferroelectric polarizations. By using asymmetric polar interfaces in the superlattices, more electrons occupy the Mn layer at the n-type interface side than at the p-type side. This charge disproportionation can be enhanced or suppressed by the ferroelectric polarization. Quantum model and density functional theory calculations reach the same conclusion: a ferromagnetic-ferrimagnetic phase transition with maximal change >90% of the total magnetization can be achieved by switching the polarization's direction. This function is robust and provides full control of the magnetization's magnitude, not only its direction, via electrical methods. C1 [Dong, Shuai] Southeast Univ, Dept Phys, Nanjing 211189, Jiangsu, Peoples R China. [Dong, Shuai; Dagotto, Elbio] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Dong, Shuai; Dagotto, Elbio] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Dong, S (reprint author), Southeast Univ, Dept Phys, Nanjing 211189, Jiangsu, Peoples R China. RI Dong (董), Shuai (帅)/A-5513-2008 OI Dong (董), Shuai (帅)/0000-0002-6910-6319 FU 973 Projects of China [2011CB922101]; NSFC [11004027, 11274060]; NCET; RFDP; U.S. DOE, Office of Basic Energy Sciences, Materials Sciences and Engineering Division FX S.D. was supported by the 973 Projects of China (2011CB922101), NSFC (11004027, 11274060), NCET, and RFDP. E.D. was supported by the U.S. DOE, Office of Basic Energy Sciences, Materials Sciences and Engineering Division. NR 40 TC 19 Z9 19 U1 1 U2 72 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 11 PY 2013 VL 88 IS 14 AR 140404 DI 10.1103/PhysRevB.88.140404 PG 5 WC Physics, Condensed Matter SC Physics GA 233GO UT WOS:000325556100001 ER PT J AU Kim, Y Strelcov, E Hwang, IR Choi, T Park, BH Jesse, S Kalinin, SV AF Kim, Yunseok Strelcov, Evgheni Hwang, In Rok Choi, Taekjib Park, Bae Ho Jesse, Stephen Kalinin, Sergei V. TI Correlative Multimodal Probing of Ionically-Mediated Electromechanical Phenomena in Simple Oxides SO SCIENTIFIC REPORTS LA English DT Article ID RESISTIVE SWITCHING MEMORIES; TRANSITION-METAL OXIDES; I-V RELATIONS; FORCE MICROSCOPY; NANOSCALE; HYSTERESIS; TRANSPORT; FERROELECTRICS; SEMICONDUCTORS; SPECTROSCOPY AB The local interplay between the ionic and electronic transport in NiO is explored using correlative imaging by first-order reversal curve measurements in current-voltage and electrochemical strain microscopy. Electronic current and electromechanical response are observed in reversible and electroforming regime. These studies provide insight into local mechanisms of electroresistive phenomena in NiO and establish universal method to study interplay between the ionic and electronic transport and electrochemical transformations in mixed electronic-ionic conductors. C1 [Kim, Yunseok; Strelcov, Evgheni; Jesse, Stephen; Kalinin, Sergei V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Kim, Yunseok] Sungkyunkwan Univ, Sch Adv Mat Sci & Engn, Suwon 440746, South Korea. [Hwang, In Rok] Konkuk Univ, Dept Phys, Div Quantum Phases & Devices, Seoul 143701, South Korea. [Hwang, In Rok; Park, Bae Ho] Korea Inst Sci & Technol, Elect Mat Res Ctr, Seoul 136791, South Korea. [Choi, Taekjib] Korea Inst Sci & Technol, Hybrid Mat Res Ctr, Seoul 136791, South Korea. [Choi, Taekjib] Korea Inst Sci & Technol, Inst Nanotechnol & Adv Mat Engn, Seoul 136791, South Korea. RP Kim, Y (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM yunseokkim@skku.edu; sergei2@ornl.gov RI Strelcov, Evgheni/H-1654-2013; Choi, Taekjib/H-8791-2012; Kalinin, Sergei/I-9096-2012; Jesse, Stephen/D-3975-2016 OI Choi, Taekjib/0000-0001-6912-3322; Kalinin, Sergei/0000-0001-5354-6152; Jesse, Stephen/0000-0002-1168-8483 FU U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division; Center for Nanophase Materials Sciences; National Laboratory by the Scientific User Facilities Division; Office of Basic Energy Sciences, U.S. Department of Energy; National Research Foundation of Korea(NRF); Korea government (MSIP) [2013R1A3A2042120]; NRF funded by the Korea MEST [2011-0025607] FX Research was supported (S.V.K., Y.K.) by the U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. A portion of this research was conducted at the Center for Nanophase Materials Sciences (S.V.K., S.J., E.S.), which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. This work was also supported by (I.R.H., B.H.P.) the National Research Foundation of Korea(NRF) grants funded by the Korea government (MSIP) (No. 2013R1A3A2042120) and (T.C.) Basic Science Research Program through the NRF funded by the Korea MEST (Grant No. 2011-0025607). NR 65 TC 14 Z9 14 U1 2 U2 61 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD OCT 11 PY 2013 VL 3 AR 2924 DI 10.1038/srep02924 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 233AN UT WOS:000325536600003 PM 24113291 ER PT J AU Milathianaki, D Boutet, S Williams, GJ Higginbotham, A Ratner, D Gleason, AE Messerschmidt, M Seibert, MM Swift, DC Hering, P Robinson, J White, WE Wark, JS AF Milathianaki, D. Boutet, S. Williams, G. J. Higginbotham, A. Ratner, D. Gleason, A. E. Messerschmidt, M. Seibert, M. M. Swift, D. C. Hering, P. Robinson, J. White, W. E. Wark, J. S. TI Femtosecond Visualization of Lattice Dynamics in Shock-Compressed Matter SO SCIENCE LA English DT Article ID METALLIZATION AB The ultrafast evolution of microstructure is key to understanding high-pressure and strain-rate phenomena. However, the visualization of lattice dynamics at scales commensurate with those of atomistic simulations has been challenging. Here, we report femtosecond x-ray diffraction measurements unveiling the response of copper to laser shock-compression at peak normal elastic stresses of similar to 73 gigapascals (GPa) and strain rates of 10(9) per second. We capture the evolution of the lattice from a one-dimensional (1D) elastic to a 3D plastically relaxed state within a few tens of picoseconds, after reaching shear stresses of 18 GPa. Our in situ high-precision measurement of material strength at spatial (<1 micrometer) and temporal (<50 picoseconds) scales provides a direct comparison with multimillion-atom molecular dynamics simulations. C1 [Milathianaki, D.; Boutet, S.; Williams, G. J.; Ratner, D.; Messerschmidt, M.; Seibert, M. M.; Hering, P.; Robinson, J.; White, W. E.] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Higginbotham, A.; Wark, J. S.] Univ Oxford, Dept Phys, Clarendon Lab, Oxford OX1 3PU, England. [Gleason, A. E.] Stanford Univ, Dept Geol & Environm Sci, Stanford, CA 94305 USA. [Seibert, M. M.] Uppsala Univ, Dept Cell & Mol Biol, S-75124 Uppsala, Sweden. [Swift, D. C.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RP Milathianaki, D (reprint author), SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. EM despina@slac.stanford.edu RI Messerschmidt, Marc/F-3796-2010 OI Messerschmidt, Marc/0000-0002-8641-3302 FU LCLS; UK Atomic Weapons Establishment; UK Engineering and Physical Sciences Research Council [EP/J017256/1] FX We thank M. Bionta, A. Fry, S. Edstrom, J. Koglin, S. Guillet, I. Ofte, and G. Stewart for assisting with our experimental requirements, data processing, and illustrations. Raw x-ray data are available upon request. This work was funded as part of the in-house research effort of LCLS, a National User Facility operated by Stanford University on behalf of the U. S. Department of Energy, Office of Basic Energy Sciences. A. H. acknowledges support from the UK Atomic Weapons Establishment and J. S. W. from the UK Engineering and Physical Sciences Research Council under grant EP/J017256/1. NR 29 TC 63 Z9 64 U1 5 U2 93 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD OCT 11 PY 2013 VL 342 IS 6155 BP 220 EP 223 DI 10.1126/science.1239566 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 232EV UT WOS:000325475200038 PM 24115435 ER PT J AU Cruz-Santiago, CA Stasto, AM AF Cruz-Santiago, C. A. Stasto, A. M. TI Recursion relations and scattering amplitudes in the light-front formalism SO NUCLEAR PHYSICS B LA English DT Article ID INFINITE-MOMENTUM; QUANTUM ELECTRODYNAMICS; DYNAMICS; GLUONS AB The fragmentation functions and scattering amplitudes are investigated in the framework of light-front perturbation theory. It is demonstrated that, the factorization property of the fragmentation functions implies the recursion relations for the off-shell scattering amplitudes which are light-front analogs of the Berends-Giele relations. These recursion relations on the light-front can be solved exactly by induction and it is shown that the expressions for the off-shell light-front amplitudes are represented as a linear combinations of the on-shell amplitudes. By putting external particles on-shell we recover the scattering amplitudes previously derived in the literature. (C) 2013 Elsevier B.V. All rights reserved. C1 [Cruz-Santiago, C. A.; Stasto, A. M.] Penn State Univ, Dept Phys, University Pk, PA 16802 USA. [Stasto, A. M.] Brookhaven Natl Lab, RIKEN Ctr, Upton, NY 11973 USA. [Stasto, A. M.] Polish Acad Sci, H Niewodniczanski Inst Nucl Phys, PL-31342 Krakow, Poland. RP Stasto, AM (reprint author), Penn State Univ, Dept Phys, 104 Davey Lab, University Pk, PA 16802 USA. EM astasto@phys.psu.edu FU DOE OJI [DE-SC0002145]; Polish NCN [DEC-2011/01/B/ST2/03915]; Sloan Foundation FX This work was supported in part by the DOE OJI grant No. DE-SC0002145 and by the Polish NCN grant DEC-2011/01/B/ST2/03915. A.M.S. is supported by the Sloan Foundation. NR 35 TC 7 Z9 7 U1 0 U2 1 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0550-3213 J9 NUCL PHYS B JI Nucl. Phys. B PD OCT 11 PY 2013 VL 875 IS 2 BP 368 EP 387 DI 10.1016/j.nuclphysb.2013.07.019 PG 20 WC Physics, Particles & Fields SC Physics GA 213TE UT WOS:000324082300003 ER PT J AU Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Rabady, D Rahbaran, B Rohringer, C Rohringer, H Schofbeck, R Strauss, J Taurok, A Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Bansal, M Bansal, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Luyckx, S Mucibello, L Ochesanu, S Roland, B Rougny, R Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Kalogeropoulos, A Keaveney, J Maes, M Olbrechts, A Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Clerbaux, B De Lentdecker, G Gay, APR Hreus, T Leonard, A Marage, PE Mohammadi, A Reis, T Thomas, L Vander Velde, C Vanlaer, P Wang, J Adler, V Beernaert, K Benucci, L Cimmino, A Costantini, S Dildick, S Garcia, G Klein, B Lellouch, J Marinov, A Mccartin, J Rios, AAO Ryckbosch, D Sigamani, M Strobbe, N Thyssen, F Tytgat, M Walsh, S Yazgan, E Zaganidis, N Basegmez, S Bruno, G Castello, R Ceard, L Delaere, C du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Lemaitre, V Liao, J Militaru, O Nuttens, C Pagano, D Pin, A Piotrzkowski, K Popov, A Selvaggi, M Garcia, JMV Beliy, N Caebergs, T Daubie, E Hammad, GH Alves, GA Martins, MC Martins, T Pol, ME Souza, MHG Alda, WL Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD De Souza, SF Malbouisson, H Malek, M Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santoro, A Jorge, LS Sznajder, A Manganote, EJT Pereira, AV Anjos, TS Bernardes, CA Dias, FA Tomei, TRFP Gregores, EM Lagana, C Marinho, F Mercadante, PC Novaes, SF Padula, SS Genchev, V Iaydjiev, P Piperov, S Rodozov, M Stoykova, S Sultanov, G Tcholakov, V Trayanov, R Vutova, M Dimitrov, A Hadjiiska, R Kozhuharov, V Litov, L Pavlov, B Petkov, P Bian, JG Chen, GM Chen, HS Jiang, CH Liang, D Liang, S Meng, X Tao, J Wang, J Wang, X Wang, Z Xiao, H Xu, M Asawatangtrakuldee, C Ban, Y Guo, Y Li, Q Li, W Liu, S Mao, Y Qian, SJ Wang, D Zhang, L Zou, W Avila, C Montoya, CAC Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Plestina, R Polic, D Puljak, I Antunovic, Z Kovac, M Brigljevic, V Dune, S Kadija, K Luetic, J Mekterovic, D Morovic, S Tikvica, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Finger, M Finger, M Assran, Y Kamel, AE Mahmoud, MA Mahrous, A Radi, A Kadastik, M Muntel, M Murumaa, M Raidal, M Rebane, L Tiko, A Eerola, P Fedi, G Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Kortelainen, MJ Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E Wendland, L Korpela, A Tuuva, T Besancon, M Choudhury, S Couderc, F Dejardin, M Denegri, D Fabbro, B Faure, JL Ferri, F Ganjour, S Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Malcles, J Millischer, L Nayak, A Rander, J Rosowsky, A Titov, M Baffioni, S Beaudette, F Benhabib, L Bianchini, L Bluj, M Busson, P Charlot, C Daci, N Dahms, T Dalchenko, M Dobrzynski, L Florent, A de Cassagnac, RG Haguenauer, M Minee, P Mironov, C Naranjo, IN Nguyen, M Ochando, C Paganini, P Sabes, D Salerno, R Sirois, Y Veelken, C Zabi, A Agram, JL Andrea, J Bloch, D Bodin, D Brom, JM Chabert, EC Collard, C Conte, E Drouhin, F Fontaine, JC Gele, D Goerlach, U Goetzmann, C Juillot, P Le Bihan, AC Van Hove, P Beauceron, S Beaupere, N Bondu, O Boudoul, G Brochet, S Chasserat, J Chierici, R Contardo, D Depasse, P El Mamouni, H Fay, J Gascon, S Gouzevitch, M Ille, B Kurca, T Lethuillier, M Mirabito, L Perries, S Sgandurra, L Sordini, V Tschudi, Y Vander Donckt, M Verdier, P Viret, S Tsamalaidze, Z Autermann, C Beranek, S Calpas, B Edelhoff, M Feld, L 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CA CMS Collaboration TI Measurement of the hadronic activity in events with a Z and two jets and extraction of the cross section for the electroweak production of a Z with two jets in pp collisions at root s=7 TeV SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering ID HIGGS-BOSON; CERN LHC AB The first measurement of the electroweak production cross section of a Z boson with two jets (Zjj) in pp collisions at root s = 7 TeV is presented, based on a data sample recorded by the CMS experiment at the LHC with an integrated luminosity of 5 fb(-1). The cross section is measured for the lljj (l = e, mu) final state in the kinematic region m(ll) > 50 GeV, m(jj) > 120 GeV, transverse momenta p(T)(j) > 25 GeV and pseudorapidity vertical bar eta(j)vertical bar < 4.0. The measurement, combining the muon and electron channels, yields sigma = 154 +/- 24 (stat.) +/- 46 (exp. syst.) +/- 27 (th. syst.) +/- 3 (lum.) fb, in agreement with the theoretical cross section. The hadronic activity, in the rapidity interval between the jets, is also measured. These results establish an important foundation for the more general study of vector boson fusion processes, of relevance for Higgs boson searches and for measurements of electroweak gauge couplings and vector boson scattering. C1 [Chatrchyan, S.; Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Bergauer, T.; Dragicevic, M.; Eroe, J.; Fabjan, C.; Friedl, M.; Fruehwirth, R.; Ghete, V. M.; Hoermann, N.; Hrubec, J.; Jeitler, M.; Kiesenhofer, W.; Knuenz, V.; Krammer, M.; Kraetschmer, I.; Liko, D.; Mikulec, I.; Rabady, D.; Rahbaran, B.; Rohringer, C.; Rohringer, H.; Schoefbeck, R.; Strauss, J.; Taurok, A.; Treberer-Treberspurg, W.; Waltenberger, W.; Wulz, C. -E.] Inst Hochenergiephys OeAW, Vienna, Austria. [Mossolov, V.; Shumeiko, N.; Gonzalez, J. Suarez] Natl Ctr Particle & High Energy Phys, Minsk, Byelarus. 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[Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Montanino, D.; Penzo, A.; Schizzi, A.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Montanino, D.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Kim, T. Y.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Chang, S.; Kim, D. H.; Kim, G. N.; Kim, J. E.; Kong, D. J.; Oh, Y. D.; Park, H.; Son, D. C.; Kamon, T.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, J. Y.; Kim, Zero J.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, T. J.; Lee, K. S.; Moon, D. H.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. S.; Kwon, E.; Lee, B.; Lee, J.; Lee, S.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Grigelionis, I.; Juodagalvis, A.] Vilnius State Univ, Vilnius, Lithuania. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Lopez-Fernandez, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.; Reyes-Santos, M. A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Bell, A. J.; Butler, P. H.; Doesburg, R.; Reucroft, S.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Asghar, M. I.; Butt, J.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bluj, M.; Bialkowska, H.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Wolszczak, W.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Almeida, N.; Bargassa, P.; David, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Kozlov, G.; Lanev, A.; Malakhov, A.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Smirnov, V.; Volodko, A.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Evstyukhin, S.; Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Matveev, V.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Erofeeva, M.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Spiridonov, A.; Stolin, V.; Toms, M.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Popov, A.; Zhukov, V.; Katkov, I.; Belyaev, A.; Boos, E.; Dubinin, M.; Ershov, A.; Khein, L.; Klyukhin, V.; Kodolova, .; Lokhtin, I.; Markina, A.; Obraztsov, S.; Petrushanko, S.; Proskuryakov, A.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia. [Adzic, P.; Ekmedzic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Ekmedzic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Alcaraz Maestre, J.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Navarro De Martino, E.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.; Willmott, C.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain. [Albajar, C.; de Troconiz, J. F.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.; Piedra Gomez, J.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Chuang, S. H.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Graziano, A.; Jorda, C.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Rabady, D.; Genchev, V.; Iaydjiev, P.; Chierici, R.; Lingemann, J.; Guthoff, M.; Hartmann, F.; Hauth, T.; Kornmayer, A.; Sharma, A.; Abdulsalam, A.; Mohanty, A. K.; Calabria, C.; De Filippis, N.; Di Matteo, L.; Gennai, S.; Lucchini, M. T.; De Cosa, A.; Meola, S.; Paolucci, P.; Bacchetta, N.; D'Agnolo, R. T.; Fiori, F.; Grassi, M.; Meridiani, P.; Mariotti, C.; Musich, M.; Cossutti, F.; Marone, M.; Seixas, J.; Kodolova, .; Chamizo Llatas, M.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Bendavid, J.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Perez, J. A. Coarasa; Colafranceschi, S.; d'Enterria, D.; Dabrowski, A.; De Roeck, A.; De Visscher, S.; Di Guida, S.; Dobson, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Eugster, J.; Funk, W.; Georgiou, G.; Giffels, M.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Giunta, M.; Glege, F.; Garrido, R. Gomez-Reino; Gowdy, S.; Guida, R.; Hammer, J.; Hansen, M.; Harris, P.; Hartl, C.; Hegner, B.; Hinzmann, A.; Innocente, V.; Janot, P.; Kaadze, K.; Karavakis, E.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lee, Y. -J.; Lourenco, C.; Magini, N.; Malberti, M.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moser, R.; Mulders, M.; Musella, P.; Nesvold, E.; Orsini, L.; Cortezon, E. Palencia; Perez, E.; Perrozzi, L.; Petrilli, A.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Piparo, D.; Polese, G.; Quertenmont, L.; Racz, A.; Reece, W.; Antunes, J. Rodrigues; Rolandi, G.; Rovelli, C.; Rovere, M.; Sakulin, H.; Santanastasio, F.; Schaefer, C.; Schwick, C.; Segoni, I.; Sekmen, S.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Stoye, M.; Tsirou, A.; Veres, G. I.; Vlimant, J. R.; Woehri, H. K.; Worm, S. D.; Zeuner, W. D.; Adiguzel, A.; Apresyan, A.; Apyan, A.; Anastassov, A.; Adair, A.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Gabathuler, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Meier, F.; Renker, D.; Rohe, T.; Naegeli, C.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bortignon, P.; Buchmann, M. A.; Casal, B.; Chanon, N.; Deisher, A.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eller, P.; Grab, C.; Hits, D.; Lecomte, P.; Lustermann, W.; Marini, A. C.; del Arbol, P. Martinez Ruiz; Mohr, N.; Moortgat, F.; Naegeli, C.; Nef, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pape, L.; Pauss, F.; Peruzzi, M.; Ronga, F. J.; Rossini, M.; Sala, L.; Sanchez, A. K.; Starodumov, A.; Stieger, B.; Takahashi, M.; Tauscher, L.; Thea, A.; Theofilatos, K.; Treille, D.; Urscheler, C.; Wallny, R.; Weber, H. A.] ETH, Inst Particle Phys, Zurich, Switzerland. [Amsler, C.; Chiochia, V.; Favaro, C.; Rikova, M. Ivova; Kilminster, B.; Mejias, B. Millan; Otiougova, P.; Robmann, P.; Snoek, H.; Taroni, S.; Tupputi, S.; Verzetti, M.] Univ Zurich, Zurich, Switzerland. [Kodolova, .; Cardaci, M.; Chen, K. H.; Ferro, C.; Kuo, C. M.; Li, S. W.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Dietz, C.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Suwonjandee, N.] Chulalongkorn Univ, Bangkok, Thailand. [Kodolova, .; Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Karapinar, G.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey. [Bahtiyar, H.; Barlas, E.; Cankocak, K.; Gunaydin, Y. O.; Vardarli, F. I.; Yucel, M.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Kreczko, L.; Metson, S.; Newbold, D. M.; Nirunpong, K.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Belyaev, A.; Worm, S. D.; Newbold, D. M.; Basso, L.; Bell, K. W.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Jackson, J.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Womersley, W. J.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Bainbridge, R.; Ball, G.; Buchmuller, O.; Burton, D.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.; Whyntie, T.] Univ London Imperial Coll Sci Technol & Med, London, England. [Chadwick, M.; Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; St John, J.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Bhattacharya, S.; Alimena, J.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Houtz, R.; Ko, W.; Kopecky, A.; Lander, R.; Mall, O.; Miceli, T.; Nelson, R.; Pellett, D.; Ricci-Tam, F.; Rutherford, B.; Searle, M.; Smith, J.; Squires, M.; Tripathi, M.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Weber, M.; Andreev, V.; Cline, D.; Cousins, R.; Erhan, S.; Everaerts, P.; Farrell, C.; Felcini, M.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Rakness, G.; Schlein, P.; Traczyk, P.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Liu, H.; Babb, J.; Clare, R.; Dinardo, M. E.; Ellison, J.; Gary, J. W.; Giordano, F.; Hanson, G.; Long, O. R.; Luthra, A.; Nguyen, H.; Paramesvaran, S.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sharma, V.; Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; Evans, D.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Macneill, I.; Mangano, B.; Padhi, S.; Palmer, C.; Petrucciani, G.; Pieri, M.; Sani, M.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Kodolova, .; Barge, D.; Bellan, R.; Campagnari, C.; D'Alfonso, M.; Danielson, T.; Flowers, K.; Geffert, P.; George, C.; Golf, F.; Incandela, J.; Justus, C.; Kalavase, P.; Kovalskyi, D.; Krutelyov, V.; Lowette, S.; Villalba, R. Magana; Mccoll, N.; Pavlunin, V.; Ribnik, J.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dias, F. A.; Dubinin, M.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Di Marco, E.; Duarte, J.; Kcira, D.; Ma, Y.; Mott, A.; Newman, H. B.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Veverka, J.; Wilkinson, R.; Xie, S.; Yang, Y.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Liu, Y. F.; Paulini, M.; Russ, J.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Nauenberg, U.; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Eggert, N.; Gibbons, L. K.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Kodolova, .; Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Gottschalk, E.; Gray, L.; Green, D.; Gutsche, O.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Klima, B.; Kunori, S.; Kwan, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Wu, W.; Yang, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Chen, M.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Drozdetskiy, A.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Remington, R.; Rinkevicius, A.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Hewamanage, S.; Lebolo, L. M.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Gleyzer, S. V.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Callner, J.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Kurt, P.; Lacroix, F.; O'Brien, C.; Silkworth, C.; Strom, D.; Turner, P.; Varelas, N.] UIC, Chicago, IL USA. [Kodolova, .; Ozturk, S.; Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Griffiths, S.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Newsom, C. R.; Ogul, H.; Onel, Y.; Ozok, F.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. 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Gomez; Goncharov, M.; Kim, Y.; Klute, M.; Levin, A.; Luckey, P. D.; Ma, T.; Nahn, S.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Sung, K.; Velicanu, D.; Wolf, R.; Wyslouch, B.; Yang, M.; Yilmaz, Y.; Yoon, A. S.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Kodolova, .; Dahmes, B.; De Benedetti, A.; Franzoni, G.; Gude, A.; Haupt, J.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Sasseville, M.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Cremaldi, L. M.; Kroeger, R.; Perera, L.; Rahmat, R.; Sanders, D. A.; Summers, D.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Eads, M.; Suarez, R. Gonzalez; Keller, J.; Kravchenko, I.; Lazo-Flores, J.; Malik, S.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. 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[Bahtiyar, H.; Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Gunaydin, Y. O.] Kahramanmaras Sutcu Imam Univ, TR-46050 Kahramanmaras, Turkey. [Belyaev, A.; Basso, L.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Wasserbaech, S.] Utah Valley Univ, Orem, UT USA. [Bilki, B.] Argonne Natl Lab, Argonne, IL 60439 USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Yetkin, T.] Yildiz Tekn Univ, Istanbul, Turkey. RP Chatrchyan, S (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Lokhtin, Igor/D-7004-2012; Manganote, Edmilson/K-8251-2013; Montanari, Alessandro/J-2420-2012; Cerrada, Marcos/J-6934-2014; Hill, Christopher/B-5371-2012; Venturi, Andrea/J-1877-2012; Calderon, Alicia/K-3658-2014; Novaes, Sergio/D-3532-2012; de la Cruz, Begona/K-7552-2014; Scodellaro, Luca/K-9091-2014; Josa, Isabel/K-5184-2014; Calvo Alamillo, Enrique/L-1203-2014; Menasce, Dario Livio/A-2168-2016; Rolandi, Luigi (Gigi)/E-8563-2013; Sguazzoni, Giacomo/J-4620-2015; Ligabue, Franco/F-3432-2014; Goh, Junghwan/Q-3720-2016; Ruiz, Alberto/E-4473-2011; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Tomei, Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Paganoni, Marco/A-4235-2016; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Tinoco Mendes, Andre David/D-4314-2011; Sznajder, Andre/L-1621-2016; Vilela Pereira, Antonio/L-4142-2016; Mundim, Luiz/A-1291-2012; Haj Ahmad, Wael/E-6738-2016; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Ragazzi, Stefano/D-2463-2009; Rovelli, Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Leonidov, Andrey/M-4440-2013; Andreev, Vladimir/M-8665-2015; Matorras, Francisco/I-4983-2015; TUVE', Cristina/P-3933-2015; KIM, Tae Jeong/P-7848-2015; Azarkin, Maxim/N-2578-2015; de Jesus Damiao, Dilson/G-6218-2012; Flix, Josep/G-5414-2012; Della Ricca, Giuseppe/B-6826-2013; VARDARLI, Fuat Ilkehan/B-6360-2013; Lazzizzera, Ignazio/E-9678-2015; Sen, Sercan/C-6473-2014; D'Alessandro, Raffaello/F-5897-2015; Belyaev, Alexander/F-6637-2015; Stahl, Achim/E-8846-2011; Trocsanyi, Zoltan/A-5598-2009; Konecki, Marcin/G-4164-2015; Hernandez Calama, Jose Maria/H-9127-2015; Bedoya, Cristina/K-8066-2014; My, Salvatore/I-5160-2015; Paulini, Manfred/N-7794-2014; Vogel, Helmut/N-8882-2014; Ferguson, Thomas/O-3444-2014; Benussi, Luigi/O-9684-2014; Russ, James/P-3092-2014; Leonidov, Andrey/P-3197-2014; vilar, rocio/P-8480-2014; da Cruz e Silva, Cristovao/K-7229-2013; Grandi, Claudio/B-5654-2015; Chinellato, Jose Augusto/I-7972-2012; Petrushanko, Sergey/D-6880-2012; Bernardes, Cesar Augusto/D-2408-2015; Raidal, Martti/F-4436-2012 OI Montanari, Alessandro/0000-0003-2748-6373; Cerrada, Marcos/0000-0003-0112-1691; Hill, Christopher/0000-0003-0059-0779; Novaes, Sergio/0000-0003-0471-8549; Scodellaro, Luca/0000-0002-4974-8330; Calvo Alamillo, Enrique/0000-0002-1100-2963; Demaria, Natale/0000-0003-0743-9465; Covarelli, Roberto/0000-0003-1216-5235; Ciulli, Vitaliano/0000-0003-1947-3396; Fiorendi, Sara/0000-0003-3273-9419; Martelli, Arabella/0000-0003-3530-2255; Gonzi, Sandro/0000-0003-4754-645X; Levchenko, Petr/0000-0003-4913-0538; Heath, Helen/0000-0001-6576-9740; Boccali, Tommaso/0000-0002-9930-9299; Menasce, Dario Livio/0000-0002-9918-1686; Attia Mahmoud, Mohammed/0000-0001-8692-5458; Bilki, Burak/0000-0001-9515-3306; Rolandi, Luigi (Gigi)/0000-0002-0635-274X; Sguazzoni, Giacomo/0000-0002-0791-3350; Casarsa, Massimo/0000-0002-1353-8964; Ligabue, Franco/0000-0002-1549-7107; Diemoz, Marcella/0000-0002-3810-8530; Tricomi, Alessia Rita/0000-0002-5071-5501; Heredia De La Cruz, Ivan/0000-0002-8133-6467; Ghezzi, Alessio/0000-0002-8184-7953; bianco, stefano/0000-0002-8300-4124; Goh, Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Vieira de Castro Ferreira da Silva, Pedro Manuel/0000-0002-5725-041X; Bean, Alice/0000-0001-5967-8674; Longo, Egidio/0000-0001-6238-6787; Di Matteo, Leonardo/0000-0001-6698-1735; Baarmand, Marc/0000-0002-9792-8619; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Paganoni, Marco/0000-0003-2461-275X; Gulmez, Erhan/0000-0002-6353-518X; Tinoco Mendes, Andre David/0000-0001-5854-7699; Sznajder, Andre/0000-0001-6998-1108; Vilela Pereira, Antonio/0000-0003-3177-4626; Mundim, Luiz/0000-0001-9964-7805; Haj Ahmad, Wael/0000-0003-1491-0446; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Ragazzi, Stefano/0000-0001-8219-2074; Rovelli, Tiziano/0000-0002-9746-4842; Matorras, Francisco/0000-0003-4295-5668; TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; de Jesus Damiao, Dilson/0000-0002-3769-1680; Flix, Josep/0000-0003-2688-8047; Della Ricca, Giuseppe/0000-0003-2831-6982; Lazzizzera, Ignazio/0000-0001-5092-7531; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Belyaev, Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279; Konecki, Marcin/0000-0001-9482-4841; Hernandez Calama, Jose Maria/0000-0001-6436-7547; Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Ferguson, Thomas/0000-0001-5822-3731; Benussi, Luigi/0000-0002-2363-8889; Russ, James/0000-0001-9856-9155; Grandi, Claudio/0000-0001-5998-3070; Chinellato, Jose Augusto/0000-0002-3240-6270; FU BMWF (Austria); FWF (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MEYS (Bulgaria); CERN (China); CAS (China); MoST (China); NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); MoER [SF0690030s09]; ERDF (Estonia); Academy of Finland (Finland); MEC (Finland); HIP (Finland); CEA (France); CNRS/IN2P3 (France); BMBF (Germany); DFG (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NKTH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF (Republic of Korea); WCU (Republic of Korea); LAS (Lithuania); CINVESTAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); MST (New Zealand); PAEC (Pakistan); MSHE (Poland); NSC (Poland); FCT (Portugal); JINR (Armenia, Belarus, Georgia, Ukraine, Uzbekistan); MON (Russia); RosAtom (Russia); RAS (Russia); RFBR (Russia); MSTD (Serbia); SEIDI (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); ThEPCenter (Thailand); IPST (Thailand); NSTDA (Thailand); TUBITAK (Turkey); TAEK (Turkey); NASU (Ukraine); STFC (United Kingdom); DOE (USA); NSF (USA); Marie-Curie programme; European Research Council; EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of Czech Republic; Council of Science and Industrial Research, India; Compagnia di San Paolo (Torino); HOMING PLUS programme of Foundation for Polish Science; EU, Regional Development Fund; Thalis programme; EU-ESF; Greek NSRF; Aristeia programme FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWF and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MEYS (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); MoER, SF0690030s09 and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NKTH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF and WCU (Republic of Korea); LAS (Lithuania); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MST (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Armenia, Belarus, Georgia, Ukraine, Uzbekistan); MON, RosAtom, RAS and RFBR (Russia); MSTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); ThEPCenter, IPST and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU (Ukraine); STFC (United Kingdom); DOE and NSF (USA).; Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of Czech Republic; the Council of Science and Industrial Research, India; the Compagnia di San Paolo (Torino); the HOMING PLUS programme of Foundation for Polish Science, co-financed by EU, Regional Development Fund; and the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF. NR 48 TC 1 Z9 1 U1 4 U2 52 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD OCT 10 PY 2013 IS 10 AR 062 DI 10.1007/JHEP10(2013)062 PG 43 WC Physics, Particles & Fields SC Physics GA AD1XT UT WOS:000333027700001 ER PT J AU Mongodin, EF Casjens, SR Bruno, JF Xu, Y Drabek, EF Riley, DR Cantarel, BL Pagan, PE Hernandez, YA Vargas, LC Dunn, JJ Schutzer, SE Fraser, CM Qiu, WG Luft, BJ AF Mongodin, Emmanuel F. Casjens, Sherwood R. Bruno, John F. Xu, Yun Drabek, Elliott Franco Riley, David R. Cantarel, Brandi L. Pagan, Pedro E. Hernandez, Yozen A. Vargas, Levy C. Dunn, John J. Schutzer, Steven E. Fraser, Claire M. Qiu, Wei-Gang Luft, Benjamin J. TI Inter- and intra-specific pan-genomes of Borrelia burgdorferi sensu lato: genome stability and adaptive radiation SO BMC GENOMICS LA English DT Article DE Borrelia burgdorferi; Lyme borreliosis; Pan-genome; Single-nucleotide polymorphisms; Phylogenetic tree; Genome evolution simulation ID LYME-DISEASE SPIROCHETE; NORTHEASTERN UNITED-STATES; FRAGMENT-LENGTH-POLYMORPHISM; MULTILOCUS SEQUENCE-ANALYSIS; FIELD GEL-ELECTROPHORESIS; SURFACE PROTEIN-C; IXODES-SCAPULARIS; NORTH-AMERICA; SP-NOV; PHYLOGENETIC ANALYSIS AB Background: Lyme disease is caused by spirochete bacteria from the Borrelia burgdorferi sensu lato (B. burgdorferi s.l.) species complex. To reconstruct the evolution of B. burgdorferi s.l. and identify the genomic basis of its human virulence, we compared the genomes of 23 B. burgdorferi s.l. isolates from Europe and the United States, including B. burgdorferi sensu stricto (B. burgdorferi s.s., 14 isolates), B. afzelii (2), B. garinii (2), B. "bavariensis" (1), B. spielmanii (1), B. valaisiana (1), B. bissettii (1), and B. "finlandensis" (1). Results: Robust B. burgdorferi s.s. and B. burgdorferi s.l. phylogenies were obtained using genome-wide single-nucleotide polymorphisms, despite recombination. Phylogeny-based pan-genome analysis showed that the rate of gene acquisition was higher between species than within species, suggesting adaptive speciation. Strong positive natural selection drives the sequence evolution of lipoproteins, including chromosomally-encoded genes 0102 and 0404, cp26-encoded ospC and b08, and lp54-encoded dbpA, a07, a22, a33, a53, a65. Computer simulations predicted rapid adaptive radiation of genomic groups as population size increases. Conclusions: Intra-and inter-specific pan-genome sizes of B. burgdorferi s.l. expand linearly with phylogenetic diversity. Yet gene-acquisition rates in B. burgdorferi s.l. are among the lowest in bacterial pathogens, resulting in high genome stability and few lineage-specific genes. Genome adaptation of B. burgdorferi s.l. is driven predominantly by copy-number and sequence variations of lipoprotein genes. New genomic groups are likely to emerge if the current trend of B. burgdorferi s.l. population expansion continues. C1 [Mongodin, Emmanuel F.; Drabek, Elliott Franco; Riley, David R.; Cantarel, Brandi L.; Fraser, Claire M.] Univ Maryland, Sch Med, Inst Genome Sci, Baltimore, MD 21201 USA. [Casjens, Sherwood R.] Univ Utah, Sch Med, Dept Pathol, Div Microbiol & Immunol, Salt Lake City, UT 84112 USA. [Bruno, John F.; Xu, Yun; Luft, Benjamin J.] SUNY Stony Brook, Hlth Sci Ctr, Dept Med, Stony Brook, NY 11794 USA. [Pagan, Pedro E.; Hernandez, Yozen A.; Vargas, Levy C.; Qiu, Wei-Gang] CUNY Hunter Coll, Dept Biol Sci, New York, NY 10065 USA. [Dunn, John J.] Brookhaven Natl Lab, Dept Biol, Upton, NY 11793 USA. [Schutzer, Steven E.] Univ Med & Dent New Jersey, New Jersey Med Sch, Dept Med, Newark, NJ 07103 USA. RP Mongodin, EF (reprint author), Univ Maryland, Sch Med, Inst Genome Sci, Baltimore, MD 21201 USA. EM emongodin@som.umaryland.edu; weigang@genectr.hunter.cuny.edu; bluft@notes.cc.sunysb.edu OI Luft, Benjamin/0000-0001-9008-7004; Fraser, Claire/0000-0003-1462-2428 FU National Institute of Allergy and Infectious Diseases (NIAID) [AI49003, AI074825, AI37256, AI107955, AI47553, N01-AI30071]; National Institute on Minority Health and Health Disparities (NIMHD) of the National Institutes of Health (NIH) [MD007599] FX This work was supported by grants AI49003, AI074825, AI37256, AI107955, AI47553 and N01-AI30071 from the National Institute of Allergy and Infectious Diseases (NIAID), and MD007599 (Hunter College) from the National Institute on Minority Health and Health Disparities (NIMHD) of the National Institutes of Health (NIH). The content of this manuscript is solely the responsibility of the authors and do not necessarily represent the official views of NIAID, NIMHD, or NIH. NR 127 TC 21 Z9 21 U1 0 U2 20 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1471-2164 J9 BMC GENOMICS JI BMC Genomics PD OCT 10 PY 2013 VL 14 AR 693 DI 10.1186/1471-2164-14-693 PG 25 WC Biotechnology & Applied Microbiology; Genetics & Heredity SC Biotechnology & Applied Microbiology; Genetics & Heredity GA 274UF UT WOS:000328631000001 PM 24112474 ER PT J AU Peukert, SL Michael, JV AF Peukert, S. L. Michael, J. V. TI High-Temperature Shock Tube and Modeling Studies on the Reactions of Methanol with D-Atoms and CH3-Radicals SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID THERMAL RATE CONSTANTS; PRESSURE RATE-CONSTANT; MULTIPASS ABSORPTION; DECOMPOSITION; DISSOCIATION; PHOTOLYSIS; PYROLYSIS; KINETICS; METHYL; FLASH AB The shock tube technique has been used to study the hydrogen abstraction reactions D + CH3OH -> CH2O + H + HD (A) and CH3 + CH3OH -> CH2O + H + CH4 (B). For reaction A, the experiments span a T-range of 1016 K <= T <= 1325 K, at pressures 0.25 bar <= P <= 0.46 bar. The experiments on reaction B, CH3 + CH3OH, cover a T-range of 1138 K <= T <= 1270 K, at pressures around 0.40 bar. Reflected shock tube experiments, monitoring the depletion of D-atoms by applying D-atom atomic resonance absorption spectrometry (ARAS), were performed on reaction A using gas mixtures of C2D5I and CH3OH in Kr bath gas. C2D5I was used as precursor for D-atoms. For reaction B, reflected shock tube experiments monitoring H-atom formation with H-ARAS, were carried out using gas mixtures of diacetyl ((CH3CO)(2)) and CH3OH in Kr bath gas. (CH3CO)(2) was used as the source of CH3-radicals. Detailed reaction models were assembled to fit the D-atom and H-atom time profiles in order to obtain experimental rate constants for reactions A and B. Total rate constants from the present experiments on D + CH3OH and CH3 + CE3OH can be represented by the Arrhenius equations k(A)(T) = 1.51 x 10(-10) exp(-3843 K/T) cm(3) molecules(-1) s(-1) (1016 K <= T <= 1325 K) and k(B)(T) = 9.62 x 10(-12) exp(-7477 KIT) cm(3) molecules(-1) s(-1) (1138 K <= T <= 1270 K). The experimentally obtained rate constants were compared with available rate data from the literature. The results from quantum chemical studies on reaction A were found to be in good agreement with the present results. The present work represents the first direct experimental study on these bimolecular reactions at combustion temperatures and is important to the high-temperature oxidation of CH3OH. C1 [Peukert, S. L.; Michael, J. V.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Michael, JV (reprint author), Argonne Natl Lab, D-183,Bldg 200, Argonne, IL 60439 USA. EM jmichael@anl.gov RI Michael, Joe/E-3907-2010 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences [DEAC02-06CH11357] FX This work was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences, under Contract No. DEAC02-06CH11357. NR 45 TC 3 Z9 3 U1 4 U2 22 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 EI 1520-5215 J9 J PHYS CHEM A JI J. Phys. Chem. A PD OCT 10 PY 2013 VL 117 IS 40 BP 10186 EP 10195 DI 10.1021/jp4059005 PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 244DI UT WOS:000326366900006 PM 23968550 ER PT J AU Peukert, SL Labbe, NJ Sivaramakrishnan, R Michael, JV AF Peukert, S. L. Labbe, N. J. Sivaramakrishnan, R. Michael, J. V. TI Direct Measurements of Rate Constants for the Reactions of CH3 Radicals with C2H6, C2H4, and C2H2 at High Temperatures SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID TRANSITION-STATE THEORY; EVALUATED KINETIC-DATA; NON-ARRHENIUS BEHAVIOR; REFLECTED SHOCK-WAVES; METHYL RADICALS; THERMAL-DECOMPOSITION; ETHYL RADICALS; H-ABSTRACTION; PYROLYSIS; HYDROGEN AB The shock tube technique has been used to study the reactions CH3 + C2H6 -> C2H4 + CH4 + H (1), CH3 + C2H4 Products + H (2), and CH3 + C2H2 -> Products + H (3). Biacetyl, (CH3CO)(2)., was used as a clean high temperature thermal source for CH3-radicals for all the three reactions studied in this work. For reaction 1, the experiments span a T-range of 1153 K <= T <= 1297 K, at P similar to 0.4 bar. The experiments on reaction 2 cover a T-range of 1176 K T 1366 K, at P similar to 1.0 bar, and those on reaction 3 a T-range of 1127 K <= T <= 1346 K, at P similar to 1.0 bar. Reflected shock tube experiments performed on reactions 1-3, monitored the formation of H-atoms with H-atom Atomic Resonance Absorption Spectrometric (ARAS). Fits to the H-atom temporal profiles using an assembled kinetics model were used to make determinations for k(1), k(2), and k(3). In the case of C2H6, the measurements of [HI-atoms were used to derive direct high-temperature rate constants, k(1), that can be represented by the Arrhenius equation k(1)(T) = 5.41 X 10(-12) exp(-6043 KIT) cm(3) molecules(-1) s(-1) (1153 K T 1297 K) for the only bimolecular process that occurs, H-atom abstraction. TST calculations based on ab initio properties calculated at the CCSD(T)/CBS/ /M06-2X/cc-pVTZ level of theory show excellent agreement, within +/- 20%, of the measured rate constants. For the reaction of CH3 with C2H4, the present rate constant results, k(2)', refer to the sum of rate constants, k(2b) + k(2c), from two competing processes, addition elimination, and the direct abstraction CH3 + C2H4 -> C3H6 + H (2b) and CH3 + C2H4 -> C2H2 + H + CH4 (2c). Experimental rate constants for k2' can be represented by the Arrhenius equation k2'(T) = 2.18 X 10(-10) exp(-11830 KIT) cm(3) molecules-1 s-1 (1176 K T 5 1366 K). The present results are in excellent agreement with recent theoretical predictions. The present study provides the only direct measurement for the high-temperature rate constants for these channels. Lastly, measurements of H-atoms from the reaction of CH3 with C2H2 provided direct unambiguous determinations of the rate constant for the dominant process under the present experimental conditions, the addition elimination, CH3 + C2H2 -> p-C3H4 + H (3b). Experimental rate constants for k(3b) can be represented by the Arrhenius equation k3b(T) = 5.16 x 10(-13) exp(-3852 KIT) cm(3) molecules(-1) s(-1) (1127 K T 1346 K). The present determinations for k3b represent the only direct measurements for this reaction and are also in good agreement with recent theoretical predictions. The present experimental k3b values were also used to derive rate constants, k(-3b), for the more extensively studied back-process, the reaction of H-atoms with propyne. The best fit Arrhenius equation, combining the presently derived k(-3b) values with a recent experimental determination for k(-3b), can be represented by k(-3b)(T) = 3. 87 x 10(-11) exp(-1313 K/T) cm(3) molecules(-1) s(-1) (870 K <= T <= 1346 K). The present studies represent a novel implementation of the sensitive H-ARAS technique to measure rate constants for poorly characterized and difficult to isolate "slow" CH3-radical reactions with stable C-2 hydrocarbons. C1 [Peukert, S. L.; Labbe, N. J.; Sivaramakrishnan, R.; Michael, J. V.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Sivaramakrishnan, R (reprint author), Argonne Natl Lab, D-183,Bldg 200, Argonne, IL 60439 USA. EM raghu@anl.gov; jmichael@anl.gov RI Michael, Joe/E-3907-2010; SIVARAMAKRISHNAN, RAGHU/C-3481-2008 OI SIVARAMAKRISHNAN, RAGHU/0000-0002-1867-1254 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences [DE-AC02-06CH11357]; Argonne-Sandia Consortium on High-Pressure Combustion Chemistry, FWP [2009 ANL 59044] FX This work was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences, under Contract No. DE-AC02-06CH11357. Support for RS. and partial support for J.V.M. was provided as part of the Argonne-Sandia Consortium on High-Pressure Combustion Chemistry, FWP# 2009 ANL 59044. NR 62 TC 2 Z9 2 U1 3 U2 31 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 EI 1520-5215 J9 J PHYS CHEM A JI J. Phys. Chem. A PD OCT 10 PY 2013 VL 117 IS 40 BP 10228 EP 10238 DI 10.1021/jp4073153 PG 11 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 244DI UT WOS:000326366900010 PM 23968575 ER PT J AU Lewandowska-Andralojc, A Polyansky, DE AF Lewandowska-Andralojc, A. Polyansky, D. E. TI Mechanism of the Quenching of the Tris(bipyridine)ruthenium(II) Emission by Persulfate: Implications for Photoinduced Oxidation Reactions SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID DRIVEN WATER OXIDATION; INDUCED ELECTRON-TRANSFER; AQUEOUS-SOLUTION; PEROXYDISULFATE ION; COMPLEXES; CATALYST; LIGANDS; PHOTOCHEMISTRY; RUTHENIUM(II); REDUCTION AB A revised mechanism for the oxidation of the excited state of Ru(bpy)(3)(2+) with the persulfate anion is described in this work. The formation of the precursor complex in the electron transfer reaction involves ion pairing between the metal complex in ground and excited states and S2O82-. The equilibrium constant for the ion-pair formation (K-IP = 2.7 M-1) was determined from electrochemical measurements and analysis of thermal reaction between Ru(bpy)(3)(2+) and persulfate. It was found to be consistent with the calculated value estimated from the Debye-Huckel model. The analysis of rate constants for reactions between persulfate and various metal complexes indicates that thermal and photochemical reactions most likely proceed through a common pathway. Extremely high reorganization energy (ca. 3.54 eV) for the electron transfer obtained from fitting experimental data with the Marcus equation is indicative of significant nuclear reorganization during the electron transfer step. In view of these results the electron transfer can be described as dissociative probably involving substantial elongation or complete scission of the O-O bond. The proposed model accurately describes experimental results for the quenching of *Ru(bpy)(3)(2+) over a wide range of persulfate concentrations and resolves some discrepancies between the values of K-IP and k(et) previously reported. The implications of various factors such as the ionic strength and dielectric constant of the medium are discussed in relation to measurements of the quantum yields in photodriven oxidation reactions employing the Ru(bpy)(3)(2+)/persulfate couple. C1 [Lewandowska-Andralojc, A.; Polyansky, D. E.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. RP Polyansky, DE (reprint author), Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. RI Lewandowska-Andralojc, Anna/A-8149-2012; Polyansky, Dmitry/C-1993-2009 OI Polyansky, Dmitry/0000-0002-0824-2296 FU U.S. Department of Energy, Division of Chemical Sciences, Geosciences, & Biosciences, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX The authors thank Dr. Norman Sutin and late Dr. Carol Creutz for very helpful discussions. We also thank Dr. James Muckerman for assistance with the DFT calculations. The work at Brookhaven National Laboratory (BNL) was carried out under contract DE-AC02-98CH10886 with the U.S. Department of Energy and supported by its Division of Chemical Sciences, Geosciences, & Biosciences, Office of Basic Energy Sciences. NR 40 TC 23 Z9 23 U1 4 U2 52 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 EI 1520-5215 J9 J PHYS CHEM A JI J. Phys. Chem. A PD OCT 10 PY 2013 VL 117 IS 40 BP 10311 EP 10319 DI 10.1021/jp407573d PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 244DI UT WOS:000326366900018 PM 24040757 ER PT J AU Pelzer, AW Jellinek, J Jackson, KA AF Pelzer, Adam W. Jellinek, Julius Jackson, Koblar A. TI H-2 Reactions on Palladium Clusters SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID MINIMUM ENERGY PATHS; SMALL METAL-CLUSTERS; ELASTIC BAND METHOD; HYDROGEN ADSORPTION; PHOTOELECTRON-SPECTROSCOPY; ELECTRONIC-STRUCTURE; CH4 ACTIVATION; SADDLE-POINTS; PD-4 CLUSTER; PEROXIDE AB Adsorption of an H-2 molecule on Pd-N clusters (N = 2-4, 7, 13, 19, and 55) is investigated using density functional theory with the hybrid PBE0 functional. Low-energy Pd-N isomers, taken from a large pool of candidate structures for all cluster sizes (except N = 55), are used in systematic searches for the most stable PdNH2 (molecular) and Pd(N)2H (dissociative) adsorption complexes. Molecular adsorption of H-2 is found to occur strictly at atop sites, with the strongest binding typically occurring at the site with the smallest coordination. Binding of dissociated H atoms occurs preferentially on 3-fold faces and on certain favorable edge sites, while binding at atop sites is unstable. Dissociative adsorption is energetically preferred to molecular adsorption for all cluster sizes. The dissociative adsorption energy decreases with cluster size, with pronounced variations due to cluster size effects for the smallest clusters. Adsorption reaction pathways are computed for cluster sizes up to N = 13. Molecular adsorption is found to be barrierless in all cases. Dissociative adsorption occurs without a barrier for the pathways studied for N = 7 and 13 and with a small barrier on the smaller clusters. Finally, lowest-energy pathways for the migration of a dissociated hydrogen atom between local minima on a cluster surface are computed for the Pd-4, Pd-7, and Pd-13 clusters. Calculated migration barriers range from 0.05 to 0.25 eV. C1 [Pelzer, Adam W.; Jellinek, Julius] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Pelzer, Adam W.; Jackson, Koblar A.] Cent Michigan Univ, Dept Phys, Mt Pleasant, MI 48859 USA. [Pelzer, Adam W.; Jackson, Koblar A.] Northwestern Univ, Dept Chem & Biol Engn, Evanston, IL 60208 USA. RP Pelzer, AW (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM adam.pelzer@northwestern.edu; jellinek@anl.gov; jackslka@cmich.edu OI Jackson, Koblar/0000-0002-5342-7978 FU U.S. Department of Energy [DE-SC0001330]; Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences, U.S. Department of Energy [DE-AC02-06CH11357]; Institute for Atom-efficient Chemical Transformations (IACT), an Energy Frontier Research Center; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences FX The authors gratefully acknowledge CMU undergraduate student Katelyn Montgomery for her assistance with aspects of this project. A.P. and K.A.J. were supported by the U.S. Department of Energy under Award No. DE-SC0001330. J.J. was supported by the Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences, U.S. Department of Energy, under Contract No. DE-AC02-06CH11357, and by the Institute for Atom-efficient Chemical Transformations (IACT), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. NR 43 TC 11 Z9 11 U1 1 U2 38 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD OCT 10 PY 2013 VL 117 IS 40 BP 10407 EP 10415 DI 10.1021/jp403089x PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 244DI UT WOS:000326366900026 PM 23980821 ER PT J AU Gong, Y Hu, HS Rao, LF Li, J Gibson, JK AF Gong, Yu Hu, Han-Shi Rao, Linfeng Li, Jun Gibson, John K. TI Experimental and Theoretical Studies on the Fragmentation of Gas-Phase Uranyl-, Neptunyl-, and Plutonyl-Diglycolamide Complexes SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID COORDINATION-COMPLEXES; RADIOLYTIC STABILITY; ACTINIDE SEPARATIONS; RADIATION-CHEMISTRY; TRANSITION-METAL; ELEMENTS 1-118; BASIS-SETS; EXTRACTION; LIGANDS; DIAMIDE AB Fragmentation of actinyl(VI) complexes (UO2)-O-VI(L)(2)(2+), (NpO2)-O-VI(L)(2)(2+), and (PuO2)-O-VI(L)(2)(2+) (L = tetramethyl-3-oxa-glutaramide, TMOGA) produced by electrospray ionization was examined in the gas phase by collision induced dissociation (CID) in a quadrupole ion trap mass spectrometer. Cleavage of the C-O-ether bond was observed for all three complexes, with dominant products being (UO2)-O-VI(L)(L-86)(+) with charge reduction, and NPv102(L)(1--101)2+ and (PuO2)-O-VI(L)(L-101)(2+) with charge conservation. The neptunyl and plutonyl complexes also exhibited substantial L+ loss to give pentavalent complexes (NpO2)-O-V(L)(+) and (PuO2)-O-V(L)(+), whereas the uranyl complex did not, consistent with the comparative An 5f-orbital energies and the An(VI)O(2)(2+)/An(V)O(2)(+) (An = U, Np, Pu) reduction potentials. CID of (NpO2)-O-V(L)(2)(+) and (PuO2)-O-V(L)(2)(+) was dominated by neutral ligand loss to form (NpO2)-O-V(L)(+) and (PuO2)-O-V(L)(+), which hydrated by addition of residual water in the ion trap; (UO2)-O-V(L)(2)(+) was not observed. Theoretical calculations of the structures and bonding of the An(VI)O(2)(L)(2)(2+) complexes using density functional, theory reveal that the metal centers are coordinated by six oxygen atoms from two TMOGA ligands. C1 [Gong, Yu; Rao, Linfeng; Gibson, John K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Hu, Han-Shi; Li, Jun] Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China. [Hu, Han-Shi; Li, Jun] Tsinghua Univ, Lab Organ Optoelect & Mol Engn, Minist Educ, Beijing 100084, Peoples R China. [Li, Jun] Pacific NW Natl Lab, William R Wiley Environm Mol Sci Lab, Richland, WA 99352 USA. RP Li, J (reprint author), Tsinghua Univ, Dept Chem, Beijing 100084, Peoples R China. EM junli@tsinghua.edu.cn; jkgibson@lbl.gov RI Li, Jun/E-5334-2011 OI Li, Jun/0000-0002-8456-3980 FU U.S. Department of Energy, Office of Basic Energy Sciences, Heavy Element Chemistry, at LBNL [DE-AC02-05CH11231]; NSFC of China [20933003, 91026003]; Department of Energy's Office of Biological and Environmental Research FX This work was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Heavy Element Chemistry, at LBNL under Contract No. DE-AC02-05CH11231 [to Y.G., L.R, and J.K.G.]. The theoretical work by H.S.H and J.L. was supported by NSFC (20933003 and 91026003) of China. The calculations were done using Tsinghua National Laboratory for Information Science and Technology and using the Molecular Science Computing capability at the EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at the PNNL, a multiprogram national laboratory operated for the Department of Energy by Battelle. We are grateful to Dr. Guoxin Tian for advice and assistance. NR 48 TC 15 Z9 16 U1 2 U2 59 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD OCT 10 PY 2013 VL 117 IS 40 BP 10544 EP 10550 DI 10.1021/jp4076977 PG 7 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 244DI UT WOS:000326366900041 PM 24015813 ER PT J AU Alfonso, DR AF Alfonso, Dominic R. TI Further Theoretical Evidence for Hydrogen-Assisted CO Dissociation on Ru(0001) SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID FISCHER-TROPSCH SYNTHESIS; PHASE ATOMIC-HYDROGEN; THERMAL-DESORPTION; ULTRASOFT PSEUDOPOTENTIALS; ADSORBATE INTERACTIONS; CHEMICAL-REACTIONS; METAL SURFACES; ADSORPTION; TRANSITION; MECHANISM AB Extensive calculations based on spin-polarized density functional theory were carried out to examine how CHx are formed from the dissociation of CO on Ru(0001) in the presence of hydrogen. Common pathways, such as the direct CO dissociation and H-assisted route leading to HCO or COH, including alternative routes that involve the formation of HCOH and CH2O, were examined. The reaction energy and barrier for each elementary step were calculated. The calculations show that the carbide mechanism is not the main reaction pathway for the conversion of CO on Ru(0001). Complementary microkinetic simulations utilizing results from first-principles quantum mechanical calculations indicate that a branch starting from the hydrogenation of CO to HCOH (via COH intermediate) and subsequent C-O bond cleavage is more plausible. C1 US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. RP Alfonso, DR (reprint author), US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. EM alfonso@netl.doe.gov FU agency of the United States Government FX Valuable advice by D. Blaylock on microkinetic simulations is strongly acknowledged. The author would also like to thank D. Sorescu, John Lo, and M. Salcicioli for fruitful discussions. This report was prepared as an account of work sponsored by an agency of the United States Government. Neither the United States Government nor any agency thereof, nor any of their employees, makes any warranty, express or implied, or assumes any legal liability or responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would not infringe privately owned rights. Reference herein to any specific commercial product, process, or service by trade name, trademark, manufacturer, or otherwise does not necessarily constitute or imply its endorsement, recommendation, or favoring by the United States Government or any agency thereof. The views and opinions of author(s) expressed herein do not necessarily state or reflect those of the United States Government or any agency thereof. NR 60 TC 8 Z9 8 U1 1 U2 32 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD OCT 10 PY 2013 VL 117 IS 40 BP 20562 EP 20571 DI 10.1021/jp403828y PG 10 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 244DH UT WOS:000326366800023 ER PT J AU Cortes, R Acharya, DP Ciobanu, CV Sutter, E Sutter, P AF Cortes, R. Acharya, D. P. Ciobanu, C. V. Sutter, E. Sutter, P. TI Graphene on Ru(0001) Moire Corrugation Studied by Scanning Tunneling Microscopy on Au/Graphene/Ru(0001) Heterostructures SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; EPITAXIAL GRAPHENE; LARGE-AREA; DEPOSITION; SURFACES; GROWTH; METALS; STATE; FILMS AB Two-dimensional Au islands of different thicknesses grown on graphene/Ru(0001) were used to study the corrugation of the moire structure of graphene/Ru(0001) and discriminate between its mainly structural or electronic character. A comparison of the apparent corrugation measured by scanning tunneling microscopy (STM) for different Au thicknesses with results of elasticity theory equations applied to a gold film over a corrugated substrate shows that the corrugation observed for the graphene/Ru(0001) moire is of structural nature rather than electronic. STM showed a large value for the corrugation of the first Au monolayer on graphene/Ru(0001), similar to 1.7 angstrom; using density functional theory calculations, we explain this large corrugation of the Au monolayer as the result of a strong (weak) binding of the Au layer at the valley (hill) regions of the graphene/Ru(0001) moire structure and infer an actual corrugation of the graphene/Ru(0001) moire structure of similar to 1.2 angstrom from the measured corrugation of the Au monolayer. C1 [Cortes, R.; Acharya, D. P.; Sutter, E.; Sutter, P.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Ciobanu, C. V.] Colorado Sch Mines, Dept Mech Engn, Golden, CO 80401 USA. [Ciobanu, C. V.] Colorado Sch Mines, Mat Sci Program, Golden, CO 80401 USA. RP Sutter, P (reprint author), Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. EM psutter@bnl.gov RI Ciobanu, Cristian/B-3580-2009 FU U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886]; BNL [114940]; NSF [CMMI-0846858] FX This research has been carried out at the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract DE-AC02-98CH10886. C.V.C. was supported by Contract 114940 from BNL and by NSF Grant CMMI-0846858. The DFT calculations were performed with resources from the Golden Energy Computing Organization. We also thank Abbas Ebnonnasir for setting up the molecular statics calculations. NR 36 TC 7 Z9 7 U1 2 U2 43 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 EI 1932-7455 J9 J PHYS CHEM C JI J. Phys. Chem. C PD OCT 10 PY 2013 VL 117 IS 40 BP 20675 EP 20680 DI 10.1021/jp406415h PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 244DH UT WOS:000326366800034 ER PT J AU Fernandez-Carrion, AJ Ocana, M Florian, P Garcia-Sevillano, J Cantelar, E Fitch, AN Suchomel, MR Becerro, AI AF Fernandez-Carrion, Alberto J. Ocana, Manuel Florian, Pierre Garcia-Sevillano, Jorge Cantelar, Eugenio Fitch, Andrew N. Suchomel, Matthew R. Becerro, Ana I. TI Crystal Structure and Luminescent Properties of Eu3+-Doped A-La2Si2O7 Tetragonal Phase Stabilized by Spray Pyrolysis Synthesis SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID RARE-EARTH DISILICATES; SOL-GEL METHOD; SI-29 MAS-NMR; YTTRIUM DISILICATE; LUTETIUM PYROSILICATE; PROFILE REFINEMENT; POWDER DIFFRACTION; Y2SI2O7; PHOTOLUMINESCENCE; SPECTROSCOPY AB Pure A-La2Si2O7 powder has been synthesized through a spray pyrolysis method followed by calcination at 1100 degrees C for 15 h. The crystallographic structure, refined from the synchrotron powder diffraction pattern of the sample, showed tetragonal symmetry with space group P4(1), a = 6.83565(1) angstrom, and c = 24.84133(1) angstrom. The Si-29 and La-139 NMR spectra have been described here for the first time in the literature and could be simulated with four Si and four La resonances, respectively, in good agreement with the presence of four Si and four La crystallographic sites in the unit cell. The same synthesis method was 2 successful for the synthesis of Eu3+-doped A-La2Si2O7 (%Eu = 3-40). The analysis of the unit cell volumes indicated that Eu3+ replaces La3+ in the unit cell for all Eu3+ substitution levels investigated. However, anomalous diffraction data indicated that the La/Eu substitution mechanism was not homogeneous, but Eu much prefers to occupy the RE3 sites. The Eu-doped A-La2Si2O7 phosphors thus synthesized exhibited a strong orange-red luminescence after excitation at 393 nm. Lifetime measurements indicated that the optimum phosphor was that with an Eu3+ content of 20%, which showed a lifetime of 2.3 ms. The quantum yield of the latter was found to be 12% at 393 nm excitation. These experimental observations together with the high purity of the phase obtained by the proposed spray pyrolysis method make this material an excellent phosphor for optoelectronic applications. C1 [Fernandez-Carrion, Alberto J.; Ocana, Manuel; Becerro, Ana I.] Inst Ciencia Mat Sevilla CSIC US, Seville 41092, Spain. [Fernandez-Carrion, Alberto J.] Univ Seville, Dept Inorgan Chem, Seville, Spain. [Florian, Pierre] UPR3079 CEMHTI, CNRS, Orleans, France. [Florian, Pierre] Univ Orleans, F-45100 Orleans, France. [Garcia-Sevillano, Jorge; Cantelar, Eugenio] Univ Autonoma Madrid, Dept Fis Mat, E-28049 Madrid, Spain. [Fitch, Andrew N.] ESRF, F-38043 Grenoble, France. [Suchomel, Matthew R.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Becerro, AI (reprint author), Inst Ciencia Mat Sevilla CSIC US, Seville 41092, Spain. EM anieto@icmse.csic.es RI Florian, Pierre/C-1840-2008; Ocana, Manuel/K-3935-2014; BECERRO, ANA /K-3804-2014; Suchomel, Matthew/C-5491-2015; OI Ocana, Manuel/0000-0001-9989-606X; BECERRO, ANA /0000-0003-2243-5438; SUCHOMEL, Matthew/0000-0002-9500-5079; Fernandez Carrion, Alberto Jose/0000-0001-8320-2828; Cantelar Alcaide, Eugenio Francisco/0000-0003-4293-8331 FU F.P.D.I. grant from Junta de Andalucia; F.P.I. grant from MICINN; DGICYT [CTQ2010-14874/BQU]; MEC [MAT2012-34919]; Junta de Andalucia [JA FQM 06090]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX A.J.F.-C. gratefully acknowledges an F.P.D.I. grant from Junta de Andalucia and J.G.-S. an F.P.I. grant from MICINN. Supported by DGICYT (Project No. CTQ2010-14874/BQU), MEC (Project. MAT2012-34919), and Junta de Andalucia (JA FQM 06090). Use of the Advanced Photon Source at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. We thank the ESRF for provision of time on beamline ID31. M. Calvo is gratefully acknowledged for help with quantum yield determination. NR 53 TC 7 Z9 7 U1 4 U2 40 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 EI 1932-7455 J9 J PHYS CHEM C JI J. Phys. Chem. C PD OCT 10 PY 2013 VL 117 IS 40 BP 20876 EP 20886 DI 10.1021/jp407172z PG 11 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 244DH UT WOS:000326366800058 ER PT J AU Staals, RHJ Agari, Y Maki-Yonekura, S Zhu, YF Taylor, DW van Duijn, E Barendregt, A Vlot, M Koehorst, JJ Sakamoto, K Masuda, A Dohmae, N Schaap, PJ Doudna, JA Heck, AJR Yonekura, K van der Oost, J Shinkai, A AF Staals, Raymond H. J. Agari, Yoshihiro Maki-Yonekura, Saori Zhu, Yifan Taylor, David W. van Duijn, Esther Barendregt, Arjan Vlot, Marnix Koehorst, Jasper J. Sakamoto, Keiko Masuda, Akiko Dohmae, Naoshi Schaap, Peter J. Doudna, Jennifer A. Heck, Albert J. R. Yonekura, Koji van der Oost, John Shinkai, Akeo TI Structure and Activity of the RNA-Targeting Type III-B CRISPR-Cas Complex of Thermus thermophilus SO MOLECULAR CELL LA English DT Article ID OF-FLIGHT INSTRUMENT; MASS-SPECTROMETRY; ESCHERICHIA-COLI; SILENCING COMPLEX; ANTIVIRAL DEFENSE; IMMUNE-SYSTEM; PROTEIN; INTERFERENCE; TRANSCRIPTION; RECOGNITION AB The CRISPR-Cas system is a prokaryotic host defense system against genetic elements. The Type III-B CRISPR-Cas system of the bacterium Thermus thermophilus, the TtCmr complex, is composed of six different protein subunits (Cmr1-6) and one crRNA with a stoichiometry of Cmr1(1)2(1)3(1)4(4)5(3)6(1): crRNA(1). The TtCmr complex copurifies with crRNA species of 40 and 46 nt, originating from a distinct subset of CRISPR loci and spacers. The TtCmr complex cleaves the target RNA at multiple sites with 6 nt intervals via a 5' ruler mechanism. Electron microscopy revealed that the structure of TtCmr resembles a "sea worm" and is composed of a Cmr2-3 heterodimer "tail," a helical backbone of Cmr4 subunits capped by Cmr5 subunits, and a curled "head" containing Cmr1 and Cmr6. Despite having a backbone of only four Cmr4 subunits and being both longer and narrower, the overall architecture of TtCmr resembles that of Type I Cascade complexes. C1 [Staals, Raymond H. J.; Zhu, Yifan; Vlot, Marnix; van der Oost, John] Wageningen Univ, Dept Agrotechnol & Food Sci, Microbiol Lab, NL-6703 HB Wageningen, Netherlands. [Agari, Yoshihiro; Maki-Yonekura, Saori; Sakamoto, Keiko; Yonekura, Koji; Shinkai, Akeo] RIKEN SPring 8 Ctr, Mikazuki, Hyogo 6795148, Japan. [Taylor, David W.] Yale Univ, Sch Med, Dept Mol Biophys & Biochem, New Haven, CT 06520 USA. [Taylor, David W.; Doudna, Jennifer A.] Univ Calif San Francisco, Calif Inst Quantitat Biosci, San Francisco, CA 94158 USA. [van Duijn, Esther; Barendregt, Arjan; Heck, Albert J. R.] Univ Utrecht, Bijvoet Ctr Biomol Res, NL-3584 CH Utrecht, Netherlands. [van Duijn, Esther; Barendregt, Arjan; Heck, Albert J. R.] Univ Utrecht, Utrecht Inst Pharmaceut Sci, NL-3584 CH Utrecht, Netherlands. [Koehorst, Jasper J.; Schaap, Peter J.] Wageningen Univ, Lab Syst & Synthet Biol, NL-6703 HB Wageningen, Netherlands. [Masuda, Akiko; Dohmae, Naoshi] RIKEN, Global Res Cluster, Wako, Saitama 3510198, Japan. [Doudna, Jennifer A.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Doudna, Jennifer A.] Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA. [Doudna, Jennifer A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP van der Oost, J (reprint author), Wageningen Univ, Dept Agrotechnol & Food Sci, Microbiol Lab, NL-6703 HB Wageningen, Netherlands. EM john.vanderoost@wur.nl; akeo.shinkai@riken.jp RI Dohmae, Naoshi/C-2040-2011; Shinkai, Akeo/E-8354-2013; YONEKURA, Koji/N-5060-2015; Heck, Albert/D-7098-2011; OI Staals, Raymond/0000-0002-5741-9457; Shinkai, Akeo/0000-0002-9867-0832; Heck, Albert/0000-0002-2405-4404; Koehorst, Jasper Jan/0000-0001-8172-8981; Taylor, David/0000-0002-6198-1194 FU Ministry of Education, Culture, Sports, Science and Technology, Japan [25440013]; ALW from the Netherlands Organization for Scientific Research (N.W.O.) [820.02.003]; Netherlands Proteomics Centre FX We thank Aimi Osaki for construction of the recombinant T. thermophilus strain, Kayoko Matsumoto and Toshi Arima for purification of the Cmr proteins, Drs. Kwang Kim and Seiki Kuramitsu for identification of the Cmr subunits by the MS/MS analysis, and Aaron Jansen for his help with the activity assays. E. Nogales, H.-W. Wang, P. Grob, and T. Houweling are acknowledged for assistance with EM and image-processing. This work was supported by a Grant-in-Aid for Scientific Research (C), 25440013, from the Ministry of Education, Culture, Sports, Science and Technology, Japan (to A.S.), and by an ALW grant (820.02.003 to J.v.d.O.) from the Netherlands Organization for Scientific Research (N.W.O.). E.v.D., A.B., and A.J.R.H. were supported by the Netherlands Proteomics Centre. D.W.T. is a National Science Foundation Graduate Research Fellow, and J.A.D. is a Howard Hughes Medical Institute Investigator. NR 38 TC 81 Z9 84 U1 1 U2 31 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 1097-2765 EI 1097-4164 J9 MOL CELL JI Mol. Cell PD OCT 10 PY 2013 VL 52 IS 1 BP 135 EP 145 DI 10.1016/j.molcel.2013.09.013 PG 11 WC Biochemistry & Molecular Biology; Cell Biology SC Biochemistry & Molecular Biology; Cell Biology GA 241VC UT WOS:000326195800013 PM 24119403 ER PT J AU Aaltonen, T Amerio, S Amidei, D Anastassov, A Annovi, A Antos, J Apollinari, G Appel, JA Arisawa, T Artikov, A Asaadi, J Ashmanskas, W Auerbach, B Aurisano, A Azfar, F Badgett, W Bae, T Barbaro-Galtieri, A Barnes, VE Barnett, BA Barria, P Bartos, P Bauce, M Bedeschi, F Behari, S Bellettini, G Bellinger, J Benjamin, D Beretvas, A Bhatti, A Bland, KR Blumenfeld, B Bocci, A Bodek, A Bortoletto, D Boudreau, J Boveia, A Brigliadori, L Bromberg, C Brucken, E Budagov, J Budd, HS Burkett, K Busetto, G Bussey, P Butti, P Buzatu, A Calamba, A Camarda, S Campanelli, M Canelli, F Carls, B Carlsmith, D Carosi, R Carrillo, S Casal, B Casarsa, M Castro, A Catastini, P Cauz, D Cavaliere, V Cavalli-Sforza, M Cerri, A Cerrito, L Chen, YC Chertok, M Chiarelli, G Chlachidze, G Cho, K Chokheli, D Clark, A Clarke, C Convery, ME Conway, J Corbo, M Cordelli, M Cox, CA Cox, DJ Cremonesi, M Cruz, D Cuevas, J Culbertson, R d'Ascenzo, N Datta, M de Barbaro, P Demortier, L Deninno, M Devoto, F D'Errico, M Di Canto, A Di Ruzza, B Dittmann, JR D'Onofrio, M Donati, S Dorigo, M Driutti, A Ebina, K Edgar, R Elagin, A Erbacher, R Errede, S Esham, B Eusebi, R Farrington, S Ramos, JPF Field, R Flanagan, G Forrest, R Franklin, M Freeman, JC Frisch, H Funakoshi, Y Galloni, C Garfinkel, AF Garosi, P Gerberich, H Gerchtein, E Giagu, S Giakoumopoulou, V Gibson, K Ginsburg, CM Giokaris, N Giromini, P Giurgiu, G Glagolev, V Glenzinski, D Gold, M Goldin, D Golossanov, A Gomez, G Gomez-Ceballos, G Goncharov, M Lopez, OG Gorelov, I Goshaw, AT Goulianos, K Gramellini, E Grinstein, S Grosso-Pilcher, C Group, RC da Costa, JG Hahn, SR Han, JY Happacher, F Hara, K Hare, M Harr, RF Harrington-Taber, T Hatakeyama, K Hays, C Heinrich, J Herndon, M Hocker, A Hong, Z Hopkins, W Hou, S Hughes, RE Husemann, U Hussein, M Huston, J Introzzi, G Iori, M Ivanov, A James, E Jang, D Jayatilaka, B Jeon, EJ Jindariani, S Jones, M Joo, KK Jun, SY Junk, TR Kambeitz, M Kamon, T Karchin, PE Kasmi, A Kato, Y Ketchum, W Keung, J Kilminster, B Kim, DH Kim, HS Kim, JE Kim, MJ Kim, SB Kim, SH Kim, YK Kim, YJ Kimura, N Kirby, M Knoepfel, K Kondo, K Kong, DJ Konigsberg, J Kotwal, AV Kreps, M Kroll, J Kruse, M Kuhr, T Kurata, M Laasanen, AT Lammel, S Lancaster, M Lannon, K Latino, G Lee, HS Lee, JS Leo, S Leone, S Lewis, JD Limosani, A Lipeles, E Lister, A Liu, H Liu, Q Liu, T Lockwitz, S Loginov, A Luca, A Lucchesi, D Lueck, J Lujan, P Lukens, P Lungu, G Lys, J Lysak, R Madrak, R Maestro, P Malik, S Manca, G Manousakis-Katsikakis, A Marchese, L Margaroli, F Marino, P Martinez, M Matera, K Mattson, ME Mazzacane, A Mazzanti, P McNulty, R Mehta, A Mehtala, P Mesropian, C Miao, T Mietlicki, D Mitra, A Miyake, H Moed, S Moggi, N Moon, CS Moore, R Morello, MJ Mukherjee, A Muller, T Murat, P Mussini, M Nachtman, J Nagai, Y Naganoma, J Nakano, I Nakano, I Nett, J Neu, C Nigmanov, T Nodulman, L Noh, SY Norniella, O Oakes, L Oh, SH Oh, YD Oksuzian, I Okusawa, T Orava, R Ortolan, L Pagliarone, C Palencia, E Palni, P Papadimitriou, V Parker, W Pauletta, G Paulini, M Paus, C Phillips, TJ Piacentino, G Pianori, E Pilot, J Pitts, K Plager, C Pondrom, L Poprocki, S Potamianos, K Prokoshin, F Pranko, A Ptohos, F Punzi, G Ranjan, N Fernandez, IR Renton, P Rescigno, M Rimondi, F Ristori, L Robson, A Rodriguez, T Rolli, S Ronzani, M Roser, R Rosner, JL Ruffini, F Ruiz, A Russ, J Rusu, V Sakumoto, WK Sakurai, Y Santi, L Sato, K Saveliev, V Savoy-Navarro, A Schlabach, P Schmidt, EE Schwarz, T Scodellaro, L Scuri, F Seidel, S Seiya, Y Semenov, A Sforza, F Shalhout, SZ Shears, T Shepard, PF Shimojima, M Shochet, M Shreyber-Tecker, I Simonenko, A Sliwa, K Smith, JR Snider, FD Sorin, V Song, H Stancari, M Denis, RS Stentz, D Strologas, J Sudo, Y Sukhanov, A Suslov, I Takemasa, K Takeuchi, Y Tang, J Tecchio, M Teng, PK Thom, J Thomson, E Thukral, V Toback, D Tokar, S Tollefson, K Tomura, T Tonelli, D Torre, S Torretta, D Totaro, P Trovato, M Ukegawa, F Uozumi, S Vazquez, F Velev, G Vellidis, C Vernieri, C Vidal, M Vilar, R Vizan, J Vogel, M Volpi, G Wagner, P Wallny, R Wang, SM Waters, D Wester, WC Whiteson, D Wicklund, AB Wilbur, S Williams, HH Wilson, JS Wilson, P Winer, BL Wittich, P Wolbers, S Wolfe, H Wright, T Wu, X Wu, Z Yamamoto, K Yamato, D Yang, T Yang, UK Yang, YC Yao, WM Yeh, GP Yi, K Yoh, J Yorita, K Yoshida, T Yu, GB Yu, I Zanetti, AM Zeng, Y Zhou, C Zucchelli, S AF Aaltonen, T. Amerio, S. Amidei, D. Anastassov, A. Annovi, A. Antos, J. Apollinari, G. Appel, J. A. Arisawa, T. Artikov, A. Asaadi, J. Ashmanskas, W. Auerbach, B. Aurisano, A. Azfar, F. Badgett, W. Bae, T. Barbaro-Galtieri, A. Barnes, V. E. Barnett, B. A. Barria, P. Bartos, P. Bauce, M. Bedeschi, F. Behari, S. Bellettini, G. Bellinger, J. Benjamin, D. Beretvas, A. Bhatti, A. Bland, K. R. Blumenfeld, B. Bocci, A. Bodek, A. Bortoletto, D. Boudreau, J. Boveia, A. Brigliadori, L. Bromberg, C. Brucken, E. Budagov, J. Budd, H. S. Burkett, K. Busetto, G. Bussey, P. Butti, P. Buzatu, A. Calamba, A. Camarda, S. Campanelli, M. Canelli, F. Carls, B. Carlsmith, D. Carosi, R. Carrillo, S. Casal, B. Casarsa, M. Castro, A. Catastini, P. Cauz, D. Cavaliere, V. Cavalli-Sforza, M. Cerri, A. Cerrito, L. Chen, Y. C. Chertok, M. Chiarelli, G. Chlachidze, G. Cho, K. Chokheli, D. Clark, A. Clarke, C. Convery, M. E. Conway, J. Corbo, M. Cordelli, M. Cox, C. A. Cox, D. J. Cremonesi, M. Cruz, D. Cuevas, J. Culbertson, R. d'Ascenzo, N. Datta, M. de Barbaro, P. Demortier, L. Deninno, M. Devoto, F. D'Errico, M. Di Canto, A. Di Ruzza, B. Dittmann, J. R. D'Onofrio, M. Donati, S. Dorigo, M. Driutti, A. Ebina, K. Edgar, R. Elagin, A. Erbacher, R. Errede, S. Esham, B. Eusebi, R. Farrington, S. Ramos, J. P. Fernandez Field, R. Flanagan, G. Forrest, R. Franklin, M. Freeman, J. C. Frisch, H. Funakoshi, Y. Galloni, C. Garfinkel, A. F. Garosi, P. Gerberich, H. Gerchtein, E. Giagu, S. Giakoumopoulou, V. Gibson, K. Ginsburg, C. M. Giokaris, N. Giromini, P. Giurgiu, G. Glagolev, V. Glenzinski, D. Gold, M. Goldin, D. Golossanov, A. Gomez, G. Gomez-Ceballos, G. Goncharov, M. Lopez, O. Gonzalez Gorelov, I. Goshaw, A. T. Goulianos, K. Gramellini, E. Grinstein, S. Grosso-Pilcher, C. Group, R. C. da Costa, J. Guimaraes Hahn, S. R. Han, J. Y. Happacher, F. Hara, K. Hare, M. Harr, R. F. Harrington-Taber, T. Hatakeyama, K. Hays, C. Heinrich, J. Herndon, M. Hocker, A. Hong, Z. Hopkins, W. Hou, S. Hughes, R. E. Husemann, U. Hussein, M. Huston, J. Introzzi, G. Iori, M. Ivanov, A. James, E. Jang, D. Jayatilaka, B. Jeon, E. J. Jindariani, S. Jones, M. Joo, K. K. Jun, S. Y. Junk, T. R. Kambeitz, M. Kamon, T. Karchin, P. E. Kasmi, A. Kato, Y. Ketchum, W. Keung, J. Kilminster, B. Kim, D. H. Kim, H. S. Kim, J. E. Kim, M. J. Kim, S. B. Kim, S. H. Kim, Y. K. Kim, Y. J. Kimura, N. Kirby, M. Knoepfel, K. Kondo, K. Kong, D. J. Konigsberg, J. Kotwal, A. V. Kreps, M. Kroll, J. Kruse, M. Kuhr, T. Kurata, M. Laasanen, A. T. Lammel, S. Lancaster, M. Lannon, K. Latino, G. Lee, H. S. Lee, J. S. Leo, S. Leone, S. Lewis, J. D. Limosani, A. Lipeles, E. Lister, A. Liu, H. Liu, Q. Liu, T. Lockwitz, S. Loginov, A. Luca, A. Lucchesi, D. Lueck, J. Lujan, P. Lukens, P. Lungu, G. Lys, J. Lysak, R. Madrak, R. Maestro, P. Malik, S. Manca, G. Manousakis-Katsikakis, A. Marchese, L. Margaroli, F. Marino, P. Martinez, M. Matera, K. Mattson, M. E. Mazzacane, A. Mazzanti, P. McNulty, R. Mehta, A. Mehtala, P. Mesropian, C. Miao, T. Mietlicki, D. Mitra, A. Miyake, H. Moed, S. Moggi, N. Moon, C. S. Moore, R. Morello, M. J. Mukherjee, A. Muller, Th. Murat, P. Mussini, M. Nachtman, J. Nagai, Y. Naganoma, J. Nakano, I. Napier, A. Nett, J. Neu, C. Nigmanov, T. Nodulman, L. Noh, S. Y. Norniella, O. Oakes, L. Oh, S. H. Oh, Y. D. Oksuzian, I. Okusawa, T. Orava, R. Ortolan, L. Pagliarone, C. Palencia, E. Palni, P. Papadimitriou, V. Parker, W. Pauletta, G. Paulini, M. Paus, C. Phillips, T. J. Piacentino, G. Pianori, E. Pilot, J. Pitts, K. Plager, C. Pondrom, L. Poprocki, S. Potamianos, K. Prokoshin, F. Pranko, A. Ptohos, F. Punzi, G. Ranjan, N. Fernandez, I. Redondo Renton, P. Rescigno, M. Rimondi, F. Ristori, L. Robson, A. Rodriguez, T. Rolli, S. Ronzani, M. Roser, R. Rosner, J. L. Ruffini, F. Ruiz, A. Russ, J. Rusu, V. Sakumoto, W. K. Sakurai, Y. Santi, L. Sato, K. Saveliev, V. Savoy-Navarro, A. Schlabach, P. Schmidt, E. E. Schwarz, T. Scodellaro, L. Scuri, F. Seidel, S. Seiya, Y. Semenov, A. Sforza, F. Shalhout, S. Z. Shears, T. Shepard, P. F. Shimojima, M. Shochet, M. Shreyber-Tecker, I. Simonenko, A. Sliwa, K. Smith, J. R. Snider, F. D. Sorin, V. Song, H. Stancari, M. Denis, R. St. Stentz, D. Strologas, J. Sudo, Y. Sukhanov, A. Suslov, I. Takemasa, K. Takeuchi, Y. Tang, J. Tecchio, M. Teng, P. K. Thom, J. Thomson, E. Thukral, V. Toback, D. Tokar, S. Tollefson, K. Tomura, T. Tonelli, D. Torre, S. Torretta, D. Totaro, P. Trovato, M. Ukegawa, F. Uozumi, S. Vazquez, F. Velev, G. Vellidis, C. Vernieri, C. Vidal, M. Vilar, R. Vizan, J. Vogel, M. Volpi, G. Wagner, P. Wallny, R. Wang, S. M. Waters, D. Wester, W. C., III Whiteson, D. Wicklund, A. B. Wilbur, S. Williams, H. H. Wilson, J. S. Wilson, P. Winer, B. L. Wittich, P. Wolbers, S. Wolfe, H. Wright, T. Wu, X. Wu, Z. Yamamoto, K. Yamato, D. Yang, T. Yang, U. K. Yang, Y. C. Yao, W. -M. Yeh, G. P. Yi, K. Yoh, J. Yorita, K. Yoshida, T. Yu, G. B. Yu, I. Zanetti, A. M. Zeng, Y. Zhou, C. Zucchelli, S. CA CDF Collaboration TI Measurement of the leptonic asymmetry in t(t)over-bar events produced in p(p)over-bar collisions at root s=1.96 TeV SO PHYSICAL REVIEW D LA English DT Article ID CHARGE ASYMMETRY AB We measure the asymmetry in the charge-weighted rapidity qy(l) of the lepton in semileptonic t (t) over bar decays recorded with the CDF II detector using the full Tevatron Run II sample, corresponding to an integrated luminosity of 9: 4 fb(-1). A parametrization of the asymmetry as a function of qy(l) is used to correct for the finite acceptance of the detector and recover the production-level asymmetry. The result of A(FB)(l) = 0.094(-0.029)(+0.032) is to be compared to the standard model next-to-leading-order prediction of A(FB)(l) = 0.038 +/- 0.003. C1 [Chen, Y. C.; Hou, S.; Mitra, A.; Teng, P. K.; Wang, S. M.] Acad Sinica, Inst Phys, Taipei 11529, Taiwan. [Auerbach, B.; Gerberich, H.; Nodulman, L.; Wicklund, A. B.] Argonne Natl Lab, Argonne, IL 60439 USA. 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RP Aaltonen, T (reprint author), Univ Helsinki, Div High Energy Phys, Dept Phys, FIN-00014 Helsinki, Finland. RI Introzzi, Gianluca/K-2497-2015; Piacentino, Giovanni/K-3269-2015; Marino, Pietro/N-7030-2015; song, hao/I-2782-2012; Gorelov, Igor/J-9010-2015; Prokoshin, Fedor/E-2795-2012; maestro, paolo/E-3280-2010; Chiarelli, Giorgio/E-8953-2012; Lysak, Roman/H-2995-2014; Moon, Chang-Seong/J-3619-2014; Scodellaro, Luca/K-9091-2014; Punzi, Giovanni/J-4947-2012; Grinstein, Sebastian/N-3988-2014; Paulini, Manfred/N-7794-2014; Russ, James/P-3092-2014; vilar, rocio/P-8480-2014; Cavalli-Sforza, Matteo/H-7102-2015; Kim, Soo-Bong/B-7061-2014; Robson, Aidan/G-1087-2011 OI Introzzi, Gianluca/0000-0002-1314-2580; Piacentino, Giovanni/0000-0001-9884-2924; Marino, Pietro/0000-0003-0554-3066; song, hao/0000-0002-3134-782X; Gorelov, Igor/0000-0001-5570-0133; Prokoshin, Fedor/0000-0001-6389-5399; maestro, paolo/0000-0002-4193-1288; Chiarelli, Giorgio/0000-0001-9851-4816; Moon, Chang-Seong/0000-0001-8229-7829; Scodellaro, Luca/0000-0002-4974-8330; Punzi, Giovanni/0000-0002-8346-9052; Grinstein, Sebastian/0000-0002-6460-8694; Paulini, Manfred/0000-0002-6714-5787; Russ, James/0000-0001-9856-9155; FU U.S. Department of Energy; National Science Foundation; Italian Istituto Nazionale di Fisica Nucleare; Ministry of Education, Culture, Sports, Science and Technology of Japan; Natural Sciences and Engineering Research Council of Canada; National Science Council of the Republic of China; Swiss National Science Foundation; A.P. Sloan Foundation; Bundesministerium fur Bildung und Forschung, Germany; Korean World Class University Program, the National Research Foundation of Korea; Science and Technology Facilities Council; Royal Society, U.K.; Russian Foundation for Basic Research; Ministerio de Ciencia e Innovacion; Programa Consolider-Ingenio, Spain; Slovak RD Agency; Academy of Finland; Australian Research Council (ARC); EU community Marie Curie Fellowship [302103] FX We acknowledge the kind assistance of A. Falkowski and T. Tait in the construction of the Octet models as well as W. Bernreuther and G. Perez for helpful discussion. We thank the Fermilab staff and the technical staffs of the participating institutions for their vital contributions. This work was supported by the U.S. Department of Energy and National Science Foundation; the Italian Istituto Nazionale di Fisica Nucleare; the Ministry of Education, Culture, Sports, Science and Technology of Japan; the Natural Sciences and Engineering Research Council of Canada; the National Science Council of the Republic of China; the Swiss National Science Foundation; the A.P. Sloan Foundation; the Bundesministerium fur Bildung und Forschung, Germany; the Korean World Class University Program, the National Research Foundation of Korea; the Science and Technology Facilities Council and the Royal Society, U.K.; the Russian Foundation for Basic Research; the Ministerio de Ciencia e Innovacion, and Programa Consolider-Ingenio 2010, Spain; the Slovak R&D Agency; the Academy of Finland; the Australian Research Council (ARC); and the EU community Marie Curie Fellowship Contract No. 302103. NR 26 TC 39 Z9 39 U1 2 U2 24 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD OCT 10 PY 2013 VL 88 IS 7 AR 072003 DI 10.1103/PhysRevD.88.072003 PG 12 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 239QA UT WOS:000326039300003 ER PT J AU Chistov, R Adachi, I Aihara, H Asner, DM Aulchenko, V Aushev, T Bakich, AM Bala, A Bhardwaj, V Bhuyan, B Bondar, A Bonvicini, G Bozek, A Bracko, M Brodzicka, J Browder, TE Chekelian, V Chen, A Chen, P Cheon, BG Chilikin, K Cho, IS Cho, K Chobanova, V Choi, Y Cinabro, D Danilov, M Dolezal, Z Drutskoy, A Dutta, D Eidelman, S Epifanov, D Farhat, H Fast, JE Feindt, M Ferber, T Frey, A Gaur, V Gabyshev, N Ganguly, S Gillard, R Goh, YM Golob, B Haba, J Hara, T Hayasaka, K Hayashii, H Horii, Y Hoshi, Y Hou, WS Hyun, HJ Iijima, T Ishikawa, A Itoh, R Iwasaki, Y Julius, T Kah, DH Kang, JH Kato, E Kawasaki, T Kichimi, H Kiesling, C Kim, DY Kim, HJ Kim, JB Kim, JH Kim, KT Kim, YJ Kinoshita, K Klucar, J Ko, BR Kodys, P Korpar, S Krizan, P Kumita, T Kuzmin, A Kwon, YJ Lange, JS Lee, SH Li, J Li, Y Libby, J Liu, C Liu, Y Liventsev, D Lukin, P Matvienko, D Miyabayashi, K Miyata, H Mizuk, R Mohanty, GB Moll, A Mori, T Muramatsu, N Mussa, R Nakano, E Nakao, M Natkaniec, Z Nayak, M Nedelkovska, E Ng, C Nishida, S Nitoh, O Ogawa, S Okuno, S Olsen, SL Oswald, C Pakhlova, G Park, CW Park, H Park, HK Pestotnik, R Petric, M Piilonen, LE Ritter, M Rohrken, M Rostomyan, A Sahoo, H Saito, T Sakai, K Sakai, Y Sandilya, S Santel, D Santelj, L Sanuki, T Savinov, V Schneider, O Schnell, G Schwanda, C Semmler, D Senyo, K Seon, O Sevior, ME Shapkin, M Shen, CP Shibata, TA Shiu, JG Shwartz, B Sibidanov, A Simon, F Sohn, YS Sokolov, A Solovieva, E Staric, M Steder, M Sumihama, M Sumiyoshi, T Tamponi, U Tanida, K Tatishvili, G Teramoto, Y Uchida, M Uglov, T Unno, Y Uno, S Urquijo, P Usov, Y Vahsen, SE Van Hulse, C Vanhoefer, P Varner, G Varvell, KE Vinokurova, A Wagner, MN Wang, CH Wang, MZ Wang, P Wang, XL Watanabe, Y Williams, KM Won, E Yabsley, BD Yamaoka, J Yamashita, Y Yashchenko, S Yook, Y Yusa, Y Zhang, ZP Zhilich, V Zhulanov, V Zupanc, A AF Chistov, R. Adachi, I. Aihara, H. Asner, D. M. Aulchenko, V. Aushev, T. Bakich, A. M. Bala, A. Bhardwaj, V. Bhuyan, B. Bondar, A. Bonvicini, G. Bozek, A. Bracko, M. Brodzicka, J. Browder, T. E. Chekelian, V. Chen, A. Chen, P. Cheon, B. G. Chilikin, K. Cho, I. -S. Cho, K. Chobanova, V. Choi, Y. Cinabro, D. Danilov, M. Dolezal, Z. Drutskoy, A. Dutta, D. Eidelman, S. Epifanov, D. Farhat, H. Fast, J. E. Feindt, M. Ferber, T. Frey, A. Gaur, V. Gabyshev, N. Ganguly, S. Gillard, R. Goh, Y. M. Golob, B. Haba, J. Hara, T. Hayasaka, K. Hayashii, H. Horii, Y. Hoshi, Y. Hou, W. -S. Hyun, H. J. Iijima, T. Ishikawa, A. Itoh, R. Iwasaki, Y. Julius, T. Kah, D. H. Kang, J. H. Kato, E. Kawasaki, T. Kichimi, H. Kiesling, C. Kim, D. Y. Kim, H. J. Kim, J. B. Kim, J. H. Kim, K. T. Kim, Y. J. Kinoshita, K. Klucar, J. Ko, B. R. Kodys, P. Korpar, S. Krizan, P. Kumita, T. Kuzmin, A. Kwon, Y. -J. Lange, J. S. Lee, S. -H. Li, J. Li, Y. Libby, J. Liu, C. Liu, Y. Liventsev, D. Lukin, P. Matvienko, D. Miyabayashi, K. Miyata, H. Mizuk, R. Mohanty, G. B. Moll, A. Mori, T. Muramatsu, N. Mussa, R. Nakano, E. Nakao, M. Natkaniec, Z. Nayak, M. Nedelkovska, E. Ng, C. Nishida, S. Nitoh, O. Ogawa, S. Okuno, S. Olsen, S. L. Oswald, C. Pakhlova, G. Park, C. W. Park, H. Park, H. K. Pestotnik, R. Petric, M. Piilonen, L. E. Ritter, M. Roehrken, M. Rostomyan, A. Sahoo, H. Saito, T. Sakai, K. Sakai, Y. Sandilya, S. Santel, D. Santelj, L. Sanuki, T. Savinov, V. Schneider, O. Schnell, G. Schwanda, C. Semmler, D. Senyo, K. Seon, O. Sevior, M. E. Shapkin, M. Shen, C. P. Shibata, T. -A. Shiu, J. -G. Shwartz, B. Sibidanov, A. Simon, F. Sohn, Y. -S. Sokolov, A. Solovieva, E. Staric, M. Steder, M. Sumihama, M. Sumiyoshi, T. Tamponi, U. Tanida, K. Tatishvili, G. Teramoto, Y. Uchida, M. Uglov, T. Unno, Y. Uno, S. Urquijo, P. Usov, Y. Vahsen, S. E. Van Hulse, C. Vanhoefer, P. Varner, G. Varvell, K. E. Vinokurova, A. Wagner, M. N. Wang, C. H. Wang, M. -Z. Wang, P. Wang, X. L. Watanabe, Y. Williams, K. M. Won, E. Yabsley, B. D. Yamaoka, J. Yamashita, Y. Yashchenko, S. Yook, Y. Yusa, Y. Zhang, Z. P. Zhilich, V. Zhulanov, V. Zupanc, A. CA Belle Collaboration TI First observation of Cabibbo-suppressed Xi(0)(c) decays SO PHYSICAL REVIEW D LA English DT Article ID BARYON DECAYS; BELLE AB We report the first observation of the Cabibbo-suppressed decays Xi(0)(c) -> Xi K--(+), Xi(0)(c) -> Lambda K+K- and Xi(0)(c) -> Lambda phi, using a data sample of 711 fb(-1) collected at the Y(4S) resonance with the Belle detector at the KEKB asymmetric-energy e(+)e(-) collider. We measure the ratios of branching fractions to be B(Xi(0)(c)->Xi K--(+))/B(Xi(0)(c)->Xi(-)pi(+)) = (2.75 +/- 0.51 +/- 0.25) x 10(-2), B(Xi(0)(c)->Lambda K+K-)/B(Xi(0)(c)->Xi(-)pi(+)) = (2.86 +/- 0.61 +/- 0.37) x 10(-2) and B(Xi(0)(c)->Lambda phi)/B(Xi(0)(c)->Xi(-)pi(+)) = (3.43 +/- 0.58 +/- 0.32) X 10(-2), where the first uncertainty is statistical and the second is systematic. C1 [Schnell, G.; Van Hulse, C.] Univ Basque Country, UPV EHU, Bilbao 48080, Spain. [Oswald, C.; Urquijo, P.] Univ Bonn, D-53115 Bonn, Germany. [Aulchenko, V.; Bondar, A.; Eidelman, S.; Gabyshev, N.; Kuzmin, A.; Lukin, P.; Matvienko, D.; Shwartz, B.; Usov, Y.; Vinokurova, A.; Zhilich, V.; Zhulanov, V.] SB RAS, Budker Inst Nucl Phys, Novosibirsk 630090, Russia. [Dolezal, Z.; Kodys, P.] Charles Univ Prague, Fac Math & Phys, CR-12116 Prague, Czech Republic. [Kinoshita, K.; Liu, Y.; Santel, D.] Univ Cincinnati, Cincinnati, OH 45221 USA. [Ferber, T.; Rostomyan, A.; Steder, M.; Yashchenko, S.] DESY, D-22607 Hamburg, Germany. [Lange, J. S.; Semmler, D.; Wagner, M. N.] Univ Giessen, D-35392 Giessen, Germany. [Sumihama, M.] Gifu Univ, Gifu 5011193, Japan. [Frey, A.] Univ Gottingen, Inst Phys 2, D-37073 Gottingen, Germany. [Cheon, B. G.; Goh, Y. M.; Unno, Y.] Hanyang Univ, Seoul 133791, South Korea. [Browder, T. E.; Sahoo, H.; Vahsen, S. E.; Varner, G.; Yamaoka, J.] Univ Hawaii, Honolulu, HI 96822 USA. [Adachi, I.; Haba, J.; Hara, T.; Itoh, R.; Iwasaki, Y.; Kichimi, H.; Liventsev, D.; Nakao, M.; Nishida, S.; Sakai, K.; Sakai, Y.; Uno, S.] High Energy Accelerator Res Org KEK, Tsukuba, Ibaraki 3050801, Japan. [Schnell, G.] Ikerbasque, Bilbao 48011, Spain. [Bhuyan, B.; Dutta, D.] Indian Inst Technol Guwahati, Gauhati 781039, Assam, India. [Libby, J.; Nayak, M.] Indian Inst Technol, Madras 600036, Tamil Nadu, India. [Wang, P.] Chinese Acad Sci, Inst High Energy Phys, Beijing 100049, Peoples R China. [Schwanda, C.] Inst High Energy Phys, A-1050 Vienna, Austria. [Shapkin, M.; Sokolov, A.] Inst High Energy Phys, Protvino 142281, Russia. [Mussa, R.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Chistov, R.; Aushev, T.; Chilikin, K.; Danilov, M.; Drutskoy, A.; Mizuk, R.; Pakhlova, G.; Solovieva, E.; Uglov, T.] Inst Theoret & Expt Phys, Moscow 117218, Russia. [Bracko, M.; Golob, B.; Klucar, J.; Korpar, S.; Krizan, P.; Pestotnik, R.; Petric, M.; Santelj, L.; Staric, M.] J Stefan Inst, Ljubljana 1000, Slovenia. [Okuno, S.; Watanabe, Y.] Kanagawa Univ, Yokohama, Kanagawa 2218686, Japan. [Feindt, M.; Roehrken, M.; Zupanc, A.] Karlsruhe Inst Technol, Inst Expt Kernphys, D-76131 Karlsruhe, Germany. [Cho, K.; Kim, J. H.; Kim, Y. J.] Korea Inst Sci & Technol Informat, Taejon 305806, South Korea. [Kim, J. B.; Kim, K. T.; Ko, B. R.; Lee, S. -H.; Won, E.] Korea Univ, Seoul 136713, South Korea. [Hyun, H. J.; Kah, D. H.; Kim, H. J.; Park, H.; Park, H. K.] Kyungpook Natl Univ, Taegu 702701, South Korea. [Schneider, O.] Ecole Polytech Fed Lausanne, CH-1015 Lausanne, Switzerland. [Golob, B.; Krizan, P.] Univ Ljubljana, Fac Math & Phys, Ljubljana 1000, Slovenia. Univ Maribor, SLO-2000 Maribor, Slovenia. [Chekelian, V.; Chobanova, V.; Kiesling, C.; Moll, A.; Nedelkovska, E.; Ritter, M.; Simon, F.; Vanhoefer, P.] Max Planck Inst Phys & Astrophys, D-80805 Munich, Germany. [Julius, T.; Sevior, M. E.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Danilov, M.; Drutskoy, A.; Mizuk, R.] Moscow Phys Engn Inst, Moscow 115409, Russia. [Uglov, T.] Moscow Inst Phys & Technol, Dolgoprudnyi 141700, Russia. [Iijima, T.; Mori, T.; Seon, O.; Shen, C. P.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648602, Japan. [Hayasaka, K.; Horii, Y.; Iijima, T.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648602, Japan. [Bhardwaj, V.; Hayashii, H.; Miyabayashi, K.] Nara Womens Univ, Nara 6308506, Japan. [Chen, A.] Natl Cent Univ, Chungli 32054, Taiwan. [Wang, C. H.] Natl United Univ, Miaoli 36003, Taiwan. [Chen, P.; Hou, W. -S.; Shiu, J. -G.; Wang, M. -Z.] Natl Taiwan Univ, Dept Phys, Taipei 10617, Taiwan. [Bozek, A.; Brodzicka, J.; Natkaniec, Z.] H Niewodniczanski Inst Nucl Phys, PL-31342 Krakow, Poland. [Yamashita, Y.] Nippon Dent Univ, Niigata 9518580, Japan. [Kawasaki, T.; Miyata, H.; Yusa, Y.] Niigata Univ, Niigata 9502181, Japan. [Nakano, E.; Teramoto, Y.] Osaka City Univ, Osaka 5588585, Japan. [Asner, D. M.; Fast, J. E.; Tatishvili, G.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Bala, A.] Panjab Univ, Chandigarh 160014, India. [Savinov, V.] Univ Pittsburgh, Pittsburgh, PA 15260 USA. [Muramatsu, N.] Tohoku Univ, Res Ctr Elect Photon Sci, Sendai, Miyagi 9808578, Japan. [Liu, C.; Zhang, Z. P.] Univ Sci & Technol China, Hefei 230026, Peoples R China. [Li, J.; Olsen, S. L.; Tanida, K.] Seoul Natl Univ, Seoul 151742, South Korea. [Kim, D. Y.] Soongsil Univ, Seoul 156743, South Korea. [Choi, Y.; Park, C. W.] Sungkyunkwan Univ, Suwon 440746, South Korea. [Bakich, A. M.; Sibidanov, A.; Varvell, K. E.; Yabsley, B. D.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Gaur, V.; Mohanty, G. B.; Sandilya, S.] Tata Inst Fundamental Res, Bombay 400005, Maharashtra, India. [Moll, A.; Simon, F.] Tech Univ Munich, Excellence Cluster Univ, D-85748 Garching, Germany. [Ogawa, S.] Toho Univ, Funabashi, Chiba 2748510, Japan. [Hoshi, Y.] Tohoku Gakuin Univ, Tagajo, Miyagi 9858537, Japan. [Ishikawa, A.; Kato, E.; Saito, T.; Sanuki, T.] Tohoku Univ, Sendai, Miyagi 9808578, Japan. [Aihara, H.; Epifanov, D.; Ng, C.] Univ Tokyo, Dept Phys, Tokyo 1130033, Japan. [Shibata, T. -A.; Uchida, M.] Tokyo Inst Technol, Tokyo 1528550, Japan. [Kumita, T.; Sumiyoshi, T.] Tokyo Metropolitan Univ, Tokyo 1920397, Japan. [Nitoh, O.] Tokyo Univ Agr & Technol, Koganei, Tokyo 1848588, Japan. [Tamponi, U.] Univ Turin, I-10124 Turin, Italy. [Li, Y.; Piilonen, L. E.; Wang, X. L.; Williams, K. M.] Virginia Polytech Inst & State Univ, CNP, Blacksburg, VA 24061 USA. [Bonvicini, G.; Cinabro, D.; Farhat, H.; Ganguly, S.; Gillard, R.] Wayne State Univ, Detroit, MI 48202 USA. [Senyo, K.] Yamagata Univ, Yamagata 9908560, Japan. [Cho, I. -S.; Kang, J. H.; Kwon, Y. -J.; Sohn, Y. -S.; Yook, Y.] Yonsei Univ, Seoul 120749, South Korea. RP Chistov, R (reprint author), Inst Theoret & Expt Phys, Moscow 117218, Russia. RI Nitoh, Osamu/C-3522-2013; Aihara, Hiroaki/F-3854-2010; Ishikawa, Akimasa/G-6916-2012; Uglov, Timofey/B-2406-2014; Danilov, Mikhail/C-5380-2014; Mizuk, Roman/B-3751-2014; Chilikin, Kirill/B-4402-2014; Chistov, Ruslan/B-4893-2014; Drutskoy, Alexey/C-8833-2016; Pakhlova, Galina/C-5378-2014; Solovieva, Elena/B-2449-2014 OI Aihara, Hiroaki/0000-0002-1907-5964; Uglov, Timofey/0000-0002-4944-1830; Danilov, Mikhail/0000-0001-9227-5164; Chilikin, Kirill/0000-0001-7620-2053; Chistov, Ruslan/0000-0003-1439-8390; Drutskoy, Alexey/0000-0003-4524-0422; Pakhlova, Galina/0000-0001-7518-3022; Solovieva, Elena/0000-0002-5735-4059 FU Ministry of Education, Culture, Sports, Science, and Technology (MEXT) of Japan; Japan Society for the Promotion of Science (JSPS); Tau-Lepton Physics Research Center of Nagoya University; Australian Research Council; Australian Department of Industry, Innovation, Science and Research; National Natural Science Foundation of China [10575109, 10775142, 10875115, 10825524]; Ministry of Education, Youth and Sports of the Czech Republic [LA10033, MSM0021620859]; Department of Science and Technology of India; Istituto Nazionale di Fisica Nucleare of Italy; Ministry Education Science and Technology, National Research Foundation of Korea; GSDC of the Korea Institute of Science and Technology Information; Polish Ministry of Science and Higher Education; Ministry of Education and Science of the Russian Federation; Russian Federal Agency for Atomic Energy; Slovenian Research Agency; Swiss National Science Foundation; National Science Council; Ministry of Education of Taiwan; U.S. Department of Energy; National Science Foundation; MEXT for Science Research in a Priority Area; JSPS for Creative Scientific Research FX We thank the KEKB group for the excellent operation of the accelerator; the KEK cryogenics group for the efficient operation of the solenoid; and the KEK computer group, the National Institute of Informatics, and the PNNL/EMSL computing group for valuable computing and SINET4 network support. We acknowledge support from the Ministry of Education, Culture, Sports, Science, and Technology (MEXT) of Japan, the Japan Society for the Promotion of Science (JSPS), and the Tau-Lepton Physics Research Center of Nagoya University; the Australian Research Council and the Australian Department of Industry, Innovation, Science and Research; the National Natural Science Foundation of China under Contracts No. 10575109, No. 10775142, No. 10875115 and No. 10825524; the Ministry of Education, Youth and Sports of the Czech Republic under Contracts No. LA10033 and No. MSM0021620859; the Department of Science and Technology of India; the Istituto Nazionale di Fisica Nucleare of Italy; the BK21 and WCU program of the Ministry Education Science and Technology, National Research Foundation of Korea, and GSDC of the Korea Institute of Science and Technology Information; the Polish Ministry of Science and Higher Education; the Ministry of Education and Science of the Russian Federation and the Russian Federal Agency for Atomic Energy; the Slovenian Research Agency; the Swiss National Science Foundation; the National Science Council and the Ministry of Education of Taiwan; and the U.S. Department of Energy and the National Science Foundation. This work is supported by a Grant-in-Aid from MEXT for Science Research in a Priority Area ("New Development of Flavor Physics"), and from JSPS for Creative Scientific Research ("Evolution of Tau-lepton Physics"). NR 15 TC 2 Z9 2 U1 1 U2 21 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD OCT 10 PY 2013 VL 88 IS 7 AR 071103 DI 10.1103/PhysRevD.88.071103 PG 7 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 239QA UT WOS:000326039300002 ER PT J AU Ivanov, AN Pitschmann, M Troitskaya, NI AF Ivanov, A. N. Pitschmann, M. Troitskaya, N. I. TI Neutron beta(-) decay as a laboratory for testing the standard model SO PHYSICAL REVIEW D LA English DT Article ID ALPHA RADIATIVE-CORRECTIONS; TIME-REVERSAL VIOLATION; EFFECTIVE-FIELD THEORY; ELECTROMAGNETIC SIMULATION; SEMILEPTONIC DECAYS; POLARIZED NEUTRONS; COULOMB CORRECTIONS; GAUGE-MODEL; LOW-ENERGY; GA-GV AB We analyze the sensitivity of all experimentally observable asymmetries and energy distributions for the neutron beta(-) decay with a polarized neutron and an unpolarized decay proton and electron, and the lifetime of the neutron to contributions of order 10(-4) of interactions beyond the standard model (SM). We analyze the contributions of interactions beyond the SM in the linear approximation with respect to the Herczeg phenomenological coupling constants, introduced at the hadronic level. Such an approximation is good enough for the analysis of contributions of order 10(-4) of interactions beyond the SM. We show that in such an approximation the correlation coefficients depend only on the axial coupling constant, which absorbs the contributions of the Herczeg left-left and left-right lepton-nucleon current-current interactions (vector and axial-vector interactions beyond the SM), and the Herczeg scalar and tensor coupling constants. In the lifetime of the neutron, in addition to the axial coupling constant, the contributions of the Herczeg left-left and left-right lepton-nucleon current-current interactions (vector and axial-vector interactions beyond the SM) are absorbed by the Cabibbo-Kobayashi-Maskawa matrix element. C1 [Ivanov, A. N.] Vienna Univ Technol, Atominst, A-1020 Vienna, Austria. [Pitschmann, M.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Pitschmann, M.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Troitskaya, N. I.] State Polytechn Univ St Petersburg, St Petersburg 195251, Russia. RP Ivanov, AN (reprint author), Vienna Univ Technol, Atominst, Stadionalle 2, A-1020 Vienna, Austria. EM ivanov@kph.tuwien.ac.at FU Austrian "Fonds zur Forderung der Wissenschaftlichen Forschung" (FWF) [I689-N16, I534-N20 PERC, I862-N20]; Russian Foundation for Basic Research [11-02-91000 -ANF_a]; U.S. Department of Energy [DE-FG02-08ER41531, DE-AC02-06CH11357]; Wisconsin Alumni Research Foundation FX We are very grateful to H. Abele and A. P. Serebrov for numerous discussions of the results obtained in this paper and for advice on the content and structure of the paper. We thank G. Konrad for discussions of the measurements of the correlation coefficient a0 by means of the measurements of the electron-proton energy distribution and the proton-energy spectrum of the neutron beta- decay. We acknowledge fruitful discussions with M. Ramsey-Musolf and M. Gonzalez-Alonso. We are grateful to W. Marciano for the discussions of the radiative corrections to the beta- decay of the neutron. We thank S. Gardner and V. Gudkov for the discussions of their results on the analysis of the beta--decay modes of the neutron, which were the foundation of our paper, as were the results obtained by Sirlin et al. This work was supported by the Austrian "Fonds zur Forderung der Wissenschaftlichen Forschung" (FWF) under Contracts No. I689-N16, No. I534-N20 PERC and No. I862-N20, by the Russian Foundation for Basic Research under Contract No. 11-02-91000 -ANF_a, and in part by the U.S. Department of Energy Contracts No. DE-FG02-08ER41531 and No. DE-AC02-06CH11357, and the Wisconsin Alumni Research Foundation. The theoretical analysis of the sensitivity of (1) the electron-proton energy distribution and the proton-energy spectrum, (2) the electron, antineutrino and proton asymmetries of correlations between the neutron spin and the 3-momenta of the decay particles and (3) the lifetime of the neutron is carried out according to the experimental program under Contract No. I534-N20 PERC, the theoretical program Contract No. I689-N16, both supported by the Austrian "Fonds zur Forderung der Wissenschaftlichen Forschung" (FWF), and the experimental program of the experimental group of the Petersburg Nuclear Physics Institute (PNPI), headed by A. P. Serebrov, under Contract No. 11-02-91000 -ANF_a, supported by the Russian Foundation for Basic Research. NR 108 TC 13 Z9 13 U1 0 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD OCT 10 PY 2013 VL 88 IS 7 AR 073002 DI 10.1103/PhysRevD.88.073002 PG 25 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 239QA UT WOS:000326039300005 ER PT J AU Lees, JP Poireau, V Tisserand, V Tico, JG Grauges, E Palano, A Eigen, G Stugu, B Brown, DN Georges, A Kerth, LT Kolomensky, YG Lynch, G Paudel, U Koch, H Schroeder, T Asgeirsson, DJ Hearty, C Mattison, TS McKenna, JA So, RY Khan, A Blinov, VE Buzykaev, AR Druzhinin, VP Golubev, VB Kravchenko, EA Onuchin, AP Serednyakov, SI Skovpen, YI Solodov, EP Todyshev, KY Yushkov, AN Bondioli, M Kirkby, D Lankford, AJ Mandelkern, M Atmacan, H Gary, JW Liu, F Long, O Vitug, GM Campagnari, C Hong, TM Kovalskyi, D Richman, JD West, CA Eisner, AM Kroseberg, J Lockman, WS Martinez, AJ Schumm, BA Seiden, A Chao, DS Cheng, CH Echenard, B Flood, KT Hitlin, DG Ongmongkolkul, P Porter, FC Rakitin, AY Andreassen, R Huard, Z Meadows, BT Sokoloff, MD Sun, L Bloom, PC Ford, WT Gaz, A Nauenberg, U Smith, JG Wagner, SR Ayad, R Toki, WH Spaan, B Schubert, KR Schwierz, R Bernard, D Verderi, M Clark, PJ Playfer, S Bettoni, D Bozzi, C Calabrese, R Cibinetto, G Fioravanti, E Garzia, I Luppi, E Munerato, M Piemontese, L Santoro, V Baldini-Ferroli, R Calcaterra, A de Sangro, R Finocchiaro, G Patteri, P Peruzzi, IM Piccolo, M Rama, M Zallo, A Contri, R Guido, E Lo Vetere, M Monge, MR Passaggio, S Patrignani, C Robutti, E Bhuyan, B Prasad, V Lee, CL Morii, M Edwards, AJ Adametz, A Uwer, U Lacker, HM Lueck, T Dauncey, PD Mallik, U Chen, C Cochran, J Meyer, WT Prell, S Rubin, AE Gritsan, AV Guo, ZJ Arnaud, N Davier, M Derkach, D Grosdidier, G Le Diberder, F Lutz, AM Malaescu, B Roudeau, P Schune, MH Stocchi, A Wormser, G Lange, DJ Wright, DM Chavez, CA Coleman, JP Fry, JR Gabathuler, E Hutchcroft, DE Payne, DJ Touramanis, C Bevan, AJ Di Lodovico, F Sacco, R Sigamani, M Cowan, G Brown, DN Davis, CL Denig, AG Fritsch, M Gradl, W Griessinger, K Hafner, A Prencipe, E Barlow, RJ Jackson, G Lafferty, GD Behn, E Cenci, R Hamilton, B Jawahery, A Roberts, DA Dallapiccola, C Cowan, R Dujmic, D Sciolla, G Cheaib, R Lindemann, D Patel, PM Robertson, SH Biassoni, P Neri, N Palombo, F Stracka, S Cremaldi, L Godang, R Kroeger, R Sonnek, P Summers, DJ Nguyen, X Simard, M Taras, P De Nardo, G Monorchio, D Onorato, G Sciacca, C Martinelli, M Raven, G Jessop, CP LoSecco, JM Wang, WF Honscheid, K Kass, R Brau, J Frey, R Sinev, NB Strom, D Torrence, E Feltresi, E Gagliardi, N Margoni, M Morandin, M Posocco, M Rotondo, M Simi, G Simonetto, F Stroili, R Akar, S Ben-Haim, E Bomben, M Bonneaud, GR Briand, H Calderini, G Chauveau, J Hamon, O Leruste, P Marchiori, G Ocariz, J Sitt, S Biasini, M Manoni, E Pacetti, S Rossi, A Angelini, C Batignani, G Bettarini, S Carpinelli, M Casarosa, G Cervelli, A Forti, F Giorgi, MA Lusiani, A Oberhof, B Paoloni, E Perez, A Rizzo, G Walsh, JJ Pegna, DL Olsen, J Smith, AJS Telnov, AV Anulli, F Faccini, R Ferrarotto, F Ferroni, F Gaspero, M Gioi, LL Mazzoni, MA Piredda, G Bunger, C Grunberg, O Hartmann, T Leddig, T Voss, C Waldi, R Adye, T Olaiya, EO Wilson, FF Emery, S de Monchenault, GH Vasseur, G Yeche, C Aston, D Bard, DJ Bartoldus, R Benitez, JF Cartaro, C Convery, MR Dorfan, J Dubois-Felsmann, GP Dunwoodie, W Ebert, M Field, RC Sevilla, MF Fulsom, BG Gabareen, AM Graham, MT Grenier, P Hast, C Innes, WR Kelsey, MH Kim, P Kocian, ML Leith, DWGS Lewis, P Lindquist, B Luitz, S Luth, V Lynch, HL MacFarlane, DB Muller, DR Neal, H Nelson, S Perl, M Pulliam, T Ratcliff, BN Roodman, A Salnikov, AA Schindler, RH Snyder, A Su, D Sullivan, MK Va'vra, J Wagner, AP Wisniewski, WJ Wittgen, M Wright, DH Wulsin, HW Young, CC Ziegler, V Park, W Purohit, MV White, RM Wilson, JR Randle-Conde, A Sekula, SJ Bellis, M Burchat, PR Miyashita, TS Puccio, EMT Alam, MS Ernst, JA Gorodeisky, R Guttman, N Peimer, DR Soffer, A Lund, P Spanier, SM Ritchie, JL Ruland, AM Schwitters, RF Wray, BC Izen, JM Lou, XC Bianchi, F Gamba, D Zambito, S Lanceri, L Vitale, L Martinez-Vidal, F Oyanguren, A Villanueva-Perez, P Ahmed, H Albert, J Banerjee, S Bernlochner, FU Choi, HHF King, GJ Kowalewski, R Lewczuk, MJ Nugent, IM Roney, JM Sobie, RJ Tasneem, N Gershon, TJ Harrison, PF Latham, TE Band, HR Dasu, S Pan, Y Prepost, R Wu, SL AF Lees, J. P. Poireau, V. Tisserand, V. Tico, J. Garra Grauges, E. Palano, A. Eigen, G. Stugu, B. Brown, D. N. Georges, A. Kerth, L. T. Kolomensky, Yu. G. Lynch, G. Paudel, U. Koch, H. Schroeder, T. Asgeirsson, D. J. Hearty, C. Mattison, T. S. McKenna, J. A. So, R. Y. Khan, A. Blinov, V. E. Buzykaev, A. R. Druzhinin, V. P. Golubev, V. B. Kravchenko, E. A. Onuchin, A. P. Serednyakov, S. I. Skovpen, Yu. I. Solodov, E. P. Todyshev, K. Yu. Yushkov, A. N. Bondioli, M. Kirkby, D. Lankford, A. J. Mandelkern, M. Atmacan, H. Gary, J. W. Liu, F. Long, O. Vitug, G. M. Campagnari, C. Hong, T. M. Kovalskyi, D. Richman, J. D. West, C. A. Eisner, A. M. Kroseberg, J. Lockman, W. S. Martinez, A. J. Schumm, B. A. Seiden, A. Chao, D. S. Cheng, C. H. Echenard, B. Flood, K. T. Hitlin, D. G. Ongmongkolkul, P. Porter, F. C. Rakitin, A. Y. Andreassen, R. Huard, Z. Meadows, B. T. Sokoloff, M. D. Sun, L. Bloom, P. C. Ford, W. T. Gaz, A. Nauenberg, U. Smith, J. G. Wagner, S. R. Ayad, R. Toki, W. H. Spaan, B. Schubert, K. R. Schwierz, R. Bernard, D. Verderi, M. Clark, P. J. Playfer, S. Bettoni, D. Bozzi, C. Calabrese, R. Cibinetto, G. Fioravanti, E. Garzia, I. Luppi, E. Munerato, M. Piemontese, L. Santoro, V. Baldini-Ferroli, R. Calcaterra, A. de Sangro, R. Finocchiaro, G. Patteri, P. Peruzzi, I. M. Piccolo, M. Rama, M. Zallo, A. Contri, R. Guido, E. Lo Vetere, M. Monge, M. R. Passaggio, S. Patrignani, C. Robutti, E. Bhuyan, B. Prasad, V. Lee, C. L. Morii, M. Edwards, A. J. Adametz, A. Uwer, U. Lacker, H. M. Lueck, T. Dauncey, P. D. Mallik, U. Chen, C. Cochran, J. Meyer, W. T. Prell, S. Rubin, A. E. Gritsan, A. V. Guo, Z. J. Arnaud, N. Davier, M. Derkach, D. Grosdidier, G. Le Diberder, F. Lutz, A. M. Malaescu, B. Roudeau, P. Schune, M. H. Stocchi, A. Wormser, G. Lange, D. J. Wright, D. M. Chavez, C. A. Coleman, J. P. Fry, J. R. Gabathuler, E. Hutchcroft, D. E. Payne, D. J. Touramanis, C. Bevan, A. J. Di Lodovico, F. Sacco, R. Sigamani, M. Cowan, G. Brown, D. N. Davis, C. L. Denig, A. G. Fritsch, M. Gradl, W. Griessinger, K. Hafner, A. Prencipe, E. Barlow, R. J. Jackson, G. Lafferty, G. D. Behn, E. Cenci, R. Hamilton, B. Jawahery, A. Roberts, D. A. Dallapiccola, C. Cowan, R. Dujmic, D. Sciolla, G. Cheaib, R. Lindemann, D. Patel, P. M. Robertson, S. H. Biassoni, P. Neri, N. Palombo, F. Stracka, S. Cremaldi, L. Godang, R. Kroeger, R. Sonnek, P. Summers, D. J. Nguyen, X. Simard, M. Taras, P. De Nardo, G. Monorchio, D. Onorato, G. Sciacca, C. Martinelli, M. Raven, G. Jessop, C. P. LoSecco, J. M. Wang, W. F. Honscheid, K. Kass, R. Brau, J. Frey, R. Sinev, N. B. Strom, D. Torrence, E. Feltresi, E. Gagliardi, N. Margoni, M. Morandin, M. Posocco, M. Rotondo, M. Simi, G. Simonetto, F. Stroili, R. Akar, S. Ben-Haim, E. Bomben, M. Bonneaud, G. R. Briand, H. Calderini, G. Chauveau, J. Hamon, O. Leruste, Ph. Marchiori, G. Ocariz, J. Sitt, S. Biasini, M. Manoni, E. Pacetti, S. Rossi, A. Angelini, C. Batignani, G. Bettarini, S. Carpinelli, M. Casarosa, G. Cervelli, A. Forti, F. Giorgi, M. A. Lusiani, A. Oberhof, B. Paoloni, E. Perez, A. Rizzo, G. Walsh, J. J. Pegna, D. Lopes Olsen, J. Smith, A. J. S. Telnov, A. V. Anulli, F. Faccini, R. Ferrarotto, F. Ferroni, F. Gaspero, M. Gioi, L. Li Mazzoni, M. A. Piredda, G. Buenger, C. Gruenberg, O. Hartmann, T. Leddig, T. Voss, C. Waldi, R. Adye, T. Olaiya, E. O. Wilson, F. F. Emery, S. de Monchenault, G. Hamel Vasseur, G. Yeche, Ch. Aston, D. Bard, D. J. Bartoldus, R. Benitez, J. F. Cartaro, C. Convery, M. R. Dorfan, J. Dubois-Felsmann, G. P. Dunwoodie, W. Ebert, M. Field, R. C. Sevilla, M. Franco Fulsom, B. G. Gabareen, A. M. Graham, M. T. Grenier, P. Hast, C. Innes, W. R. Kelsey, M. H. Kim, P. Kocian, M. L. Leith, D. W. G. S. Lewis, P. Lindquist, B. Luitz, S. Luth, V. Lynch, H. L. MacFarlane, D. B. Muller, D. R. Neal, H. Nelson, S. Perl, M. Pulliam, T. Ratcliff, B. N. Roodman, A. Salnikov, A. A. Schindler, R. H. Snyder, A. Su, D. Sullivan, M. K. Va'vra, J. Wagner, A. P. Wisniewski, W. J. Wittgen, M. Wright, D. H. Wulsin, H. W. Young, C. C. Ziegler, V. Park, W. Purohit, M. V. White, R. M. Wilson, J. R. Randle-Conde, A. Sekula, S. J. Bellis, M. Burchat, P. R. Miyashita, T. S. Puccio, E. M. T. Alam, M. S. Ernst, J. A. Gorodeisky, R. Guttman, N. Peimer, D. R. Soffer, A. Lund, P. Spanier, S. M. Ritchie, J. L. Ruland, A. M. Schwitters, R. F. Wray, B. C. Izen, J. M. Lou, X. C. Bianchi, F. Gamba, D. Zambito, S. Lanceri, L. Vitale, L. Martinez-Vidal, F. Oyanguren, A. Villanueva-Perez, P. Ahmed, H. Albert, J. Banerjee, Sw. Bernlochner, F. U. Choi, H. H. F. King, G. J. Kowalewski, R. Lewczuk, M. J. Nugent, I. M. Roney, J. M. Sobie, R. J. Tasneem, N. Gershon, T. J. Harrison, P. F. Latham, T. E. Band, H. R. Dasu, S. Pan, Y. Prepost, R. Wu, S. L. CA BABAR Collaboration TI Search for a low-mass scalar Higgs boson decaying to a tau pair in single-photon decays of Y(1S) SO PHYSICAL REVIEW D LA English DT Article ID LEPTONIC DECAYS; QUARKONIUM; DETECTOR; PARTICLE; MODEL; LHC AB We search for a low-mass scalar CP-odd Higgs boson, A(0), produced in the radiative decay of the upsilon resonance and decaying into a tau(+)tau(-) pair: Y(1S) -> gamma A(0). The production of Y(1S) mesons is tagged by Y(2S) -> pi(+)pi(-) Y(1S) transitions, using a sample of (98.3 +/- 0.9) x 10(6) Y(2S) mesons collected by the BABAR detector. We find no evidence for a Higgs boson in the mass range 3: 5 <= m(A)0 <= 9: 2 GeV, and combine these results with our previous search for the tau decays of the light Higgs in radiative Y(3S) decays, setting limits on the coupling of A(0) to the b (b) over bar quarks in the range 0.09-1.9. 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B.; Muller, D. R.; Neal, H.; Nelson, S.; Perl, M.; Pulliam, T.; Ratcliff, B. N.; Roodman, A.; Salnikov, A. A.; Schindler, R. H.; Snyder, A.; Su, D.; Sullivan, M. K.; Va'vra, J.; Wagner, A. P.; Wisniewski, W. J.; Wittgen, M.; Wright, D. H.; Wulsin, H. W.; Young, C. C.; Ziegler, V.] SLAC Natl Accelerator Lab, Stanford, CA 94309 USA. [Park, W.; Purohit, M. V.; White, R. M.; Wilson, J. R.] Univ S Carolina, Columbia, SC 29208 USA. [Randle-Conde, A.; Sekula, S. J.] So Methodist Univ, Dallas, TX 75275 USA. [Bellis, M.; Burchat, P. R.; Miyashita, T. S.; Puccio, E. M. T.] Stanford Univ, Stanford, CA 94305 USA. [Alam, M. S.; Ernst, J. A.] SUNY Albany, Albany, NY 12222 USA. [Gorodeisky, R.; Guttman, N.; Peimer, D. R.; Soffer, A.] Tel Aviv Univ, Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Lund, P.; Spanier, S. M.] Univ Tennessee, Knoxville, TN 37996 USA. [Ritchie, J. L.; Ruland, A. M.; Schwitters, R. F.; Wray, B. C.] Univ Texas Austin, Austin, TX 78712 USA. [Izen, J. M.; Lou, X. C.] Univ Texas Dallas, Richardson, TX 75083 USA. [Bianchi, F.; Gamba, D.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Bianchi, F.; Gamba, D.; Zambito, S.] Univ Turin, Dipartimento Fis Sperimentale, I-10125 Turin, Italy. [Lanceri, L.; Vitale, L.] Ist Nazl Fis Nucl, Sez Trieste, I-34127 Trieste, Italy. [Lanceri, L.; Vitale, L.] Univ Trieste, Dipartmento Fis, I-34127 Trieste, Italy. [Martinez-Vidal, F.; Oyanguren, A.; Villanueva-Perez, P.] Univ Valencia, CSIC, IFIC, E-46071 Valencia, Spain. [Ahmed, H.; Albert, J.; Banerjee, Sw.; Bernlochner, F. U.; Choi, H. H. F.; King, G. J.; Kowalewski, R.; Lewczuk, M. J.; Nugent, I. M.; Roney, J. M.; Sobie, R. J.; Tasneem, N.] Univ Victoria, Victoria, BC V8W 3P6, Canada. [Gershon, T. J.; Harrison, P. F.; Latham, T. E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Band, H. R.; Dasu, S.; Pan, Y.; Prepost, R.; Wu, S. L.] Univ Wisconsin, Madison, WI 53706 USA. [Peruzzi, I. M.] Univ Perugia, Dipartimento Fis, I-06100 Perugia, Italy. [Carpinelli, M.] Univ Sassari, I-07100 Sassari, Italy. RP Ayad, R (reprint author), Univ Tabuk, Tabuk 71491, Saudi Arabia. RI Rizzo, Giuliana/A-8516-2015; Morandin, Mauro/A-3308-2016; Lusiani, Alberto/A-3329-2016; Stracka, Simone/M-3931-2015; Di Lodovico, Francesca/L-9109-2016; Calcaterra, Alessandro/P-5260-2015; Frey, Raymond/E-2830-2016; Patrignani, Claudia/C-5223-2009; Monge, Maria Roberta/G-9127-2012; Forti, Francesco/H-3035-2011; Oyanguren, Arantza/K-6454-2014; Luppi, Eleonora/A-4902-2015; White, Ryan/E-2979-2015; Kravchenko, Evgeniy/F-5457-2015; Calabrese, Roberto/G-4405-2015; Martinez Vidal, F*/L-7563-2014; Kolomensky, Yury/I-3510-2015; Lo Vetere, Maurizio/J-5049-2012; Lusiani, Alberto/N-2976-2015 OI Pacetti, Simone/0000-0002-6385-3508; Rizzo, Giuliana/0000-0003-1788-2866; Faccini, Riccardo/0000-0003-2613-5141; Bellis, Matthew/0000-0002-6353-6043; Morandin, Mauro/0000-0003-4708-4240; Lusiani, Alberto/0000-0002-6876-3288; Stracka, Simone/0000-0003-0013-4714; Di Lodovico, Francesca/0000-0003-3952-2175; Calcaterra, Alessandro/0000-0003-2670-4826; Frey, Raymond/0000-0003-0341-2636; Paoloni, Eugenio/0000-0001-5969-8712; Bettarini, Stefano/0000-0001-7742-2998; Cibinetto, Gianluigi/0000-0002-3491-6231; Patrignani, Claudia/0000-0002-5882-1747; Monge, Maria Roberta/0000-0003-1633-3195; Forti, Francesco/0000-0001-6535-7965; Oyanguren, Arantza/0000-0002-8240-7300; Luppi, Eleonora/0000-0002-1072-5633; White, Ryan/0000-0003-3589-5900; Calabrese, Roberto/0000-0002-1354-5400; Martinez Vidal, F*/0000-0001-6841-6035; Kolomensky, Yury/0000-0001-8496-9975; Lo Vetere, Maurizio/0000-0002-6520-4480; Lusiani, Alberto/0000-0002-6876-3288 FU DOE (USA); NSF (USA); NSERC (Canada); CEA (France); CNRS-IN2P3 (France); BMBF (Germany); DFG (Germany); INFN (Italy); FOM (The Netherlands); NFR (Norway); MES (Russia); MICIIN (Spain); STFC (United Kingdom); Marie Curie EIF (European Union); A. P. Sloan Foundation (USA); Binational Science Foundation (USA-Israel) FX We are grateful for the excellent luminosity and machine conditions provided by our PEP-II colleagues, and for the substantial dedicated effort from the computing organizations that support BABAR. The collaborating institutions wish to thank SLAC for its support and kind hospitality. This work is supported by DOE and NSF (USA), NSERC (Canada), CEA and CNRS-IN2P3 (France), BMBF and DFG (Germany), INFN (Italy), FOM (The Netherlands), NFR (Norway), MES (Russia), MICIIN (Spain), and STFC (United Kingdom). Individuals have received support from the Marie Curie EIF (European Union), the A. P. Sloan Foundation (USA) and the Binational Science Foundation (USA-Israel). NR 31 TC 17 Z9 17 U1 1 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD OCT 10 PY 2013 VL 88 IS 7 AR 071102 DI 10.1103/PhysRevD.88.071102 PG 8 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 239QA UT WOS:000326039300001 ER PT J AU Prim, M Adachi, I Aihara, H Asner, DM Aushev, T Bakich, AM Bala, A Bhuyan, B Bonvicini, G Bozek, A Bracko, M Browder, TE Cervenkov, D Chang, MC Chang, P Chekelian, V Chen, A Chen, P Cheon, BG Chistov, R Cho, K Chobanova, V Choi, Y Cinabro, D Danilov, M Dolezal, Z Draal, Z Dutta, D Eidelman, S Farhat, H Feindt, M Ferber, T Frey, A Gaur, V Ganguly, S Gillard, R Goh, YM Golob, B Hayashii, H Heider, M Hoshi, Y Hou, WS Hsiung, YB Iijima, T Inami, K Ishikawa, A Itoh, R Jaegle, I Julius, T Kah, DH Kawai, H Kawasaki, T Kichimi, H Kiesling, C Kim, DY Kim, HO Kim, JB Kim, JH Kim, MJ Kim, YJ Kinoshita, K Klucar, J Ko, BR Kodys, P Krizan, P Krokovny, P Kronenbitter, B Kuhr, T Kumita, T Kwon, YJ Lange, JS Lee, SH Li, J Libby, J Lukin, P Matvienko, D Miyabayashi, K Miyata, H Mizuk, R Mohanty, GB Moll, A Muramatsu, N Mussa, R Nakamura, I Nakano, E Nakao, M Nayak, M Nedelkovska, E Niebuhr, C Nisar, NK Nishida, S Nitoh, O Onuki, Y Pakhlova, G Park, H Park, HK Pedlar, TK Pestotnik, R Petric, M Piilonen, LE Ritter, M Rohrken, M Rostomyan, A Rozanska, M Sahoo, H Saito, T Sakai, Y Sandilya, S Sanuki, T Sato, Y Savinov, V Schneider, O Schnell, G Schwanda, C Semmler, D Senyo, K Sevior, ME Shapkin, M Shen, CP Shibata, TA Shiu, JG Sibidanov, A Sohn, YS Sokolov, A Solovieva, E Staric, M Steder, M Sumiyoshi, T Tamponi, U Tatishvili, G Teramoto, Y Trabelsi, K Tsuboyama, T Uchida, M Uehara, S Uglov, T Unno, Y Uno, S Usov, Y Vahsen, SE Van Hulse, C Vanhoefer, P Varner, G Vorobyev, V Wang, CH Wang, MZ Wang, P Wang, XL Watanabe, M Watanabe, Y Williams, KM Won, E Yamashita, Y Yashchenko, S Zhang, ZP Zhilich, V Zupanc, A AF Prim, M. Adachi, I. Aihara, H. Asner, D. M. Aushev, T. Bakich, A. M. Bala, A. Bhuyan, B. Bonvicini, G. Bozek, A. Bracko, M. Browder, T. E. Cervenkov, D. Chang, M. -C. Chang, P. Chekelian, V. Chen, A. Chen, P. Cheon, B. G. Chistov, R. Cho, K. Chobanova, V. Choi, Y. Cinabro, D. Danilov, M. Dolezal, Z. Drasal, Z. Dutta, D. Eidelman, S. Farhat, H. Feindt, M. Ferber, T. Frey, A. Gaur, V. Ganguly, S. Gillard, R. Goh, Y. M. Golob, B. Hayashii, H. Heider, M. Hoshi, Y. Hou, W. -S. Hsiung, Y. B. Iijima, T. Inami, K. Ishikawa, A. Itoh, R. Jaegle, I. Julius, T. Kah, D. H. Kawai, H. Kawasaki, T. Kichimi, H. Kiesling, C. Kim, D. Y. Kim, H. O. Kim, J. B. Kim, J. H. Kim, M. J. Kim, Y. J. Kinoshita, K. Klucar, J. Ko, B. R. Kodys, P. Krizan, P. Krokovny, P. Kronenbitter, B. Kuhr, T. Kumita, T. Kwon, Y. -J. Lange, J. S. Lee, S. -H. Li, J. Libby, J. Lukin, P. Matvienko, D. Miyabayashi, K. Miyata, H. Mizuk, R. Mohanty, G. B. Moll, A. Muramatsu, N. Mussa, R. Nakamura, I. Nakano, E. Nakao, M. Nayak, M. Nedelkovska, E. Niebuhr, C. Nisar, N. K. Nishida, S. Nitoh, O. Onuki, Y. Pakhlova, G. Park, H. Park, H. K. Pedlar, T. K. Pestotnik, R. Petric, M. Piilonen, L. E. Ritter, M. Roehrken, M. Rostomyan, A. Rozanska, M. Sahoo, H. Saito, T. Sakai, Y. Sandilya, S. Sanuki, T. Sato, Y. Savinov, V. Schneider, O. Schnell, G. Schwanda, C. Semmler, D. Senyo, K. Sevior, M. E. Shapkin, M. Shen, C. P. Shibata, T. -A. Shiu, J. -G. Sibidanov, A. Sohn, Y. -S. Sokolov, A. Solovieva, E. Staric, M. Steder, M. Sumiyoshi, T. Tamponi, U. Tatishvili, G. Teramoto, Y. Trabelsi, K. Tsuboyama, T. Uchida, M. Uehara, S. Uglov, T. Unno, Y. Uno, S. Usov, Y. Vahsen, S. E. Van Hulse, C. Vanhoefer, P. Varner, G. Vorobyev, V. Wang, C. H. Wang, M. -Z. Wang, P. Wang, X. L. Watanabe, M. Watanabe, Y. Williams, K. M. Won, E. Yamashita, Y. Yashchenko, S. Zhang, Z. P. Zhilich, V. Zupanc, A. CA Belle Collaboration TI Angular analysis of B-0 -> phi K* decays and search for CP violation at Belle SO PHYSICAL REVIEW D LA English DT Article ID DETECTOR; SCATTERING; PACKAGE AB We report the measurements of branching fractions and CP violation asymmetries in B-0 -> phi K* decays obtained in an angular analysis using the full data sample of 772 x 10(6) B (B) over bar pairs collected at the Upsilon(4S) resonance with the Belle detector at the KEKB asymmetric-energy e(+)e(-) collider. We perform a partial wave analysis to distinguish among scalar [B-0 -> phi(K pi)(0)*], vector [B-0 -> phi K*(892)(0)] and tensor [B-0 -> phi K-2*(1430)(0)] components, and determine the corresponding branching fractions to be B[B-0 -> phi(K pi)(0)*] = (4.3 +/- 0.4 +/- 0.4) x 10(-6), B[B-0 -> phi K*(892)(0)] = (10.4 +/- 0.5 +/- 0.6) x 10(-6) and B[B-0 -> phi K-2*(1430)(0)] = (5.5(-0.7)(+0.9) +/- 1.0) x 10(-6). We also measure the longitudinal polarization fraction f(L) in B-0 -> phi K*(892)(0) and B-0 -> phi K-2*(1430)(0) decays to be 0.499 +/- 0.030 +/- 0.018 and 0.918(-0.060)(-0.029) +/- 0.012, respectively. The first quoted uncertainties are statistical and the second are systematic. In total, we measure 26 parameters related to branching fractions, polarization and CP violation in the B-0 -> phi K* system. No evidence for CP violation is found. C1 [Schnell, G.; Van Hulse, C.] Univ Basque Country, UPV EHU, Bilbao 48080, Spain. [Shen, C. P.] Beihang Univ, Beijing 100191, Peoples R China. [Eidelman, S.; Krokovny, P.; Lukin, P.; Matvienko, D.; Usov, Y.; Vorobyev, V.; Zhilich, V.] SB RAS, Budker Inst Nucl Phys, Novosibirsk 630090, Russia. [Cervenkov, D.; Dolezal, Z.; Drasal, Z.; Kodys, P.] Charles Univ Prague, Fac Math & Phys, CR-12116 Prague, Czech Republic. [Kawai, H.] Chiba Univ, Chiba 2638522, Japan. [Ferber, T.; Goh, Y. M.; Niebuhr, C.; Rostomyan, A.; Steder, M.; Yashchenko, S.] DESY, D-22607 Hamburg, Germany. [Chang, M. -C.] Fu Jen Catholic Univ, Dept Phys, Taipei 24205, Taiwan. [Lange, J. S.; Semmler, D.] Univ Giessen, D-35392 Giessen, Germany. [Cheon, B. G.; Unno, Y.] Hanyang Univ, Seoul 133791, South Korea. [Browder, T. E.; Jaegle, I.; Sahoo, H.; Vahsen, S. E.; Varner, G.] Univ Hawaii, Honolulu, HI 96822 USA. [Adachi, I.; Itoh, R.; Kichimi, H.; Nakamura, I.; Nakao, M.; Nishida, S.; Sakai, Y.; Trabelsi, K.; Tsuboyama, T.; Uehara, S.; Uno, S.] High Energy Accelerator Res Org KEK, Tsukuba, Ibaraki 3050801, Japan. [Schnell, G.] Basque Fdn Sci, Ikerbasque, Bilbao 48011, Spain. [Bhuyan, B.; Dutta, D.] Indian Inst Technol Guwahati, Gauhati 781039, Assam, India. [Libby, J.; Nayak, M.] Indian Inst Technol, Madras 600036, Tamil Nadu, India. [Wang, P.] Chinese Acad Sci, Inst High Energy Phys, Beijing 100049, Peoples R China. [Schwanda, C.] Inst High Energy Phys, A-1050 Vienna, Austria. [Shapkin, M.; Sokolov, A.] Inst High Energy Phys, Protvino 142281, Russia. [Mussa, R.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Aushev, T.; Chistov, R.; Danilov, M.; Mizuk, R.; Pakhlova, G.; Solovieva, E.; Uglov, T.] Inst Theoret & Expt Phys, Moscow 117218, Russia. [Bracko, M.; Golob, B.; Klucar, J.; Krizan, P.; Pestotnik, R.; Petric, M.; Staric, M.] J Stefan Inst, Ljubljana 1000, Slovenia. [Sibidanov, A.; Watanabe, Y.] Kanagawa Univ, Yokohama, Kanagawa 2218686, Japan. [Prim, M.; Feindt, M.; Heider, M.; Kronenbitter, B.; Kuhr, T.; Roehrken, M.; Zupanc, A.] Karlsruhe Inst Technol, Inst Expt Kernphys, D-76131 Karlsruhe, Germany. [Cho, K.; Kim, J. H.; Kim, Y. J.] Korea Inst Sci & Technol Informat, Taejon 305806, South Korea. [Kim, J. B.; Ko, B. R.; Lee, S. -H.; Won, E.] Korea Univ, Seoul 136713, South Korea. [Kah, D. H.; Kim, H. O.; Kim, M. J.; Park, H.; Park, H. K.] Kyungpook Natl Univ, Taegu 702701, South Korea. [Schneider, O.] Ecole Polytech Fed Lausanne, CH-1015 Lausanne, Switzerland. [Golob, B.; Krizan, P.] Univ Ljubljana, Fac Math & Phys, Ljubljana 1000, Slovenia. [Pedlar, T. K.] Luther Coll, Iowa City, IA 52101 USA. [Bracko, M.] Univ Maribor, SLO-2000 Maribor, Slovenia. [Chekelian, V.; Chobanova, V.; Kiesling, C.; Moll, A.; Nedelkovska, E.; Ritter, M.; Vanhoefer, P.] Max Planck Inst Phys & Astrophys, D-80805 Munich, Germany. [Julius, T.; Sevior, M. E.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Danilov, M.; Mizuk, R.] Moscow Engn Phys Inst, Moscow 115409, Russia. [Uglov, T.] Moscow Inst Phys & Technol, Moscow 141700, Russia. [Iijima, T.; Inami, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648602, Japan. [Iijima, T.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648602, Japan. [Chen, A.] Natl Cent Univ, Chungli 32054, Taiwan. [Wang, C. H.] Natl United Univ, Miaoli 36003, Taiwan. [Chang, P.; Chen, P.; Hou, W. -S.; Hsiung, Y. B.; Shiu, J. -G.; Wang, M. -Z.] Natl Taiwan Univ, Dept Phys, Taipei 10617, Taiwan. [Bozek, A.; Rozanska, M.] H Niewodniczanski Inst Nucl Phys, PL-31342 Krakow, Poland. [Yamashita, Y.] Nippon Dent Univ, Niigata 9518580, Japan. [Kawasaki, T.; Miyata, H.; Watanabe, M.] Niigata Univ, Niigata 9502181, Japan. [Nakano, E.; Teramoto, Y.] Osaka City Univ, Osaka 5588585, Japan. [Asner, D. M.; Tatishvili, G.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Bala, A.] Panjab Univ, Chandigarh 160014, India. [Savinov, V.] Univ Pittsburgh, Pittsburgh, PA 15260 USA. [Muramatsu, N.] Tohoku Univ, Res Ctr Elect Photon Sci, Sendai, Miyagi 9808578, Japan. [Zhang, Z. P.] Univ Sci & Technol China, Hefei 230026, Peoples R China. [Li, J.] Seoul Natl Univ, Seoul 151742, South Korea. [Kim, D. Y.] Soongsil Univ, Seoul 156743, South Korea. [Choi, Y.] Sungkyunkwan Univ, Suwon 440746, South Korea. [Bakich, A. M.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Gaur, V.; Mohanty, G. B.; Nisar, N. K.; Sandilya, S.] Tata Inst Fundamental Res, Bombay 400005, Maharashtra, India. [Moll, A.] Tech Univ Munich, Excellence Cluster Univ, D-85748 Garching, Germany. [Hoshi, Y.] Tohoku Gakuin Univ, Tagajo, Miyagi 9858537, Japan. [Ishikawa, A.; Saito, T.; Sanuki, T.; Sato, Y.] Tohoku Univ, Sendai, Miyagi 9808578, Japan. [Aihara, H.; Onuki, Y.] Univ Tokyo, Dept Phys, Tokyo 1130033, Japan. [Shibata, T. -A.; Uchida, M.] Tokyo Inst Technol, Tokyo 1528550, Japan. [Kumita, T.; Sumiyoshi, T.] Tokyo Metropolitan Univ, Tokyo 1920397, Japan. [Nitoh, O.] Tokyo Univ Agr & Technol, Koganei, Tokyo 1848588, Japan. [Tamponi, U.] Univ Turin, I-10124 Turin, Italy. [Piilonen, L. E.; Wang, X. L.; Williams, K. M.] Virginia Polytech Inst & State Univ, CNP, Blacksburg, VA 24061 USA. [Bonvicini, G.; Cinabro, D.; Farhat, H.; Ganguly, S.; Gillard, R.] Wayne State Univ, Detroit, MI 48202 USA. [Senyo, K.] Yamagata Univ, Yamagata 9908560, Japan. [Kwon, Y. -J.; Sohn, Y. -S.] Yonsei Univ, Seoul 120749, South Korea. [Frey, A.] Univ Gottingen, Inst Phys 2, D-37073 Gottingen, Germany. [Hayashii, H.; Miyabayashi, K.] Nara Womens Univ, Nara 6308506, Japan. [Kinoshita, K.] Univ Cincinnati, Cincinnati, OH 45221 USA. RP Prim, M (reprint author), Karlsruhe Inst Technol, Inst Expt Kernphys, D-76131 Karlsruhe, Germany. RI Nitoh, Osamu/C-3522-2013; Aihara, Hiroaki/F-3854-2010; Ishikawa, Akimasa/G-6916-2012; Uglov, Timofey/B-2406-2014; Danilov, Mikhail/C-5380-2014; Mizuk, Roman/B-3751-2014; Krokovny, Pavel/G-4421-2016; Chistov, Ruslan/B-4893-2014; Pakhlova, Galina/C-5378-2014; Cervenkov, Daniel/D-2884-2017; Solovieva, Elena/B-2449-2014 OI Trabelsi, Karim/0000-0001-6567-3036; Aihara, Hiroaki/0000-0002-1907-5964; Uglov, Timofey/0000-0002-4944-1830; Danilov, Mikhail/0000-0001-9227-5164; Krokovny, Pavel/0000-0002-1236-4667; Chistov, Ruslan/0000-0003-1439-8390; Pakhlova, Galina/0000-0001-7518-3022; Cervenkov, Daniel/0000-0002-1865-741X; Solovieva, Elena/0000-0002-5735-4059 FU Ministry of Education, Culture, Sports, Science, and Technology (MEXT) of Japan; Japan Society for the Promotion of Science (JSPS); Tau-Lepton Physics Research Center of Nagoya University; Australian Research Council; Australian Department of Industry, Innovation, Science and Research; Austrian Science Fund [P 22742-N16]; National Natural Science Foundation of China [10575109, 10775142, 10875115, 10825524]; Ministry of Education, Youth and Sports of the Czech Republic [MSM0021620859]; Carl Zeiss Foundation; Deutsche Forschungsgemeinschaft; VolkswagenStiftung; Department of Science and Technology of India; Istituto Nazionale di Fisica Nucleare of Italy; Ministry Education Science and Technology, National Research Foundation of Korea [2010-0021174, 2011-0029457, 2012-0008143, 2012R1A1A2008330]; BRL program under NRF [KRF-2011-0020333]; GSDC of the Korea Institute of Science and Technology Information; Polish Ministry of Science and Higher Education; National Science Center; Ministry of Education and Science of the Russian Federation; Russian Federal Agency for Atomic Energy; Slovenian Research Agency; Basque Foundation for Science (IKERBASQUE); UPV/EHU [UFI 11/55]; Swiss National Science Foundation; National Science Council; Ministry of Education of Taiwan; U. S. Department of Energy; National Science Foundation; MEXT for Science Research in a Priority Area ("New Development of Flavor Physics"); JSPS for Creative Scientific Research ("Evolution of Tau-lepton Physics") FX We thank the KEKB group for the excellent operation of the accelerator; the KEK cryogenics group for the efficient operation of the solenoid; and the KEK computer group, the National Institute of Informatics, and the PNNL/EMSL computing group for valuable computing and SINET4 network support. We acknowledge support from the Ministry of Education, Culture, Sports, Science, and Technology (MEXT) of Japan, the Japan Society for the Promotion of Science (JSPS), and the Tau-Lepton Physics Research Center of Nagoya University; the Australian Research Council and the Australian Department of Industry, Innovation, Science and Research; Austrian Science Fund under Grant No. P 22742-N16; the National Natural Science Foundation of China under Contracts No. 10575109, No. 10775142, No. 10875115 and No. 10825524; the Ministry of Education, Youth and Sports of the Czech Republic under Contract No. MSM0021620859; the Carl Zeiss Foundation, the Deutsche Forschungsgemeinschaft and the VolkswagenStiftung; the Department of Science and Technology of India; the Istituto Nazionale di Fisica Nucleare of Italy; the BK21 and WCU program of the Ministry Education Science and Technology, National Research Foundation of Korea Grants No. 2010-0021174, No. 2011-0029457, No. 2012-0008143, and No. 2012R1A1A2008330, BRL program under NRF Grant No. KRF-2011-0020333, and GSDC of the Korea Institute of Science and Technology Information; the Polish Ministry of Science and Higher Education and the National Science Center; the Ministry of Education and Science of the Russian Federation and the Russian Federal Agency for Atomic Energy; the Slovenian Research Agency; the Basque Foundation for Science (IKERBASQUE) and the UPV/EHU under program UFI 11/55; the Swiss National Science Foundation; the National Science Council and the Ministry of Education of Taiwan; and the U. S. Department of Energy and the National Science Foundation. This work is supported by a Grant-in-Aid from MEXT for Science Research in a Priority Area ("New Development of Flavor Physics"), and from JSPS for Creative Scientific Research ("Evolution of Tau-lepton Physics"). NR 33 TC 14 Z9 14 U1 2 U2 28 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD OCT 10 PY 2013 VL 88 IS 7 AR 072004 DI 10.1103/PhysRevD.88.072004 PG 15 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 239QA UT WOS:000326039300004 ER PT J AU Adriani, O Bonechi, L Bongi, M Castellini, G D'Alessandro, R Haguenauer, M Iso, T Itow, Y Kasahara, K Kawade, K Masuda, K Menjo, H Mitsuka, G Muraki, Y Noda, K Papini, P Perrot, AL Ricciarini, S Sako, T Shimizu, Y Suzuki, T Tamura, T Torii, S Tricomi, A Turner, WC AF Adriani, O. Bonechi, L. Bongi, M. Castellini, G. D'Alessandro, R. Haguenauer, M. Iso, T. Itow, Y. Kasahara, K. Kawade, K. Masuda, K. Menjo, H. Mitsuka, G. Muraki, Y. Noda, K. Papini, P. Perrot, A. -L. Ricciarini, S. Sako, T. Shimizu, Y. Suzuki, T. Tamura, T. Torii, S. Tricomi, A. Turner, W. C. CA LHCf Collaboration TI LHCf DETECTOR PERFORMANCE DURING THE 2009-2010 LHC RUN SO INTERNATIONAL JOURNAL OF MODERN PHYSICS A LA English DT Review DE LHCf; sampling calorimeter; particle identification ID GAMMA-RAY SPECTRA; PROTON-PROTON COLLISIONS; PHOTON ENERGY-SPECTRA AB Large Hadron Collider forward (LHCf) has successfully completed the operation during the LHC 2009-2010 period and the detectors were removed in July 2010. The event trigger, data analysis and background have been intensively studied in order to derive inclusive single photon and pi(0) spectra. In this paper, the details of these intensive studies are described. C1 [Adriani, O.; Bonechi, L.; Bongi, M.; Castellini, G.; D'Alessandro, R.; Menjo, H.; Papini, P.; Ricciarini, S.] Ist Nazl Fis Nucl, Sect Florence, Florence, Italy. [Adriani, O.; Bongi, M.; D'Alessandro, R.; Mitsuka, G.] Univ Florence, I-50121 Florence, Italy. [Haguenauer, M.] Ecole Polytech, Palaiseau, France. [Iso, T.; Itow, Y.; Kawade, K.; Masuda, K.; Mitsuka, G.; Muraki, Y.; Sako, T.] Nagoya Univ, Solar Terr Environm Lab, Nagoya, Aichi 4648601, Japan. [Itow, Y.; Menjo, H.; Sako, T.] Nagoya Univ, Kobayashi Maskawa Inst Origin Particles & Univers, Nagoya, Aichi 4648601, Japan. [Kasahara, K.; Shimizu, Y.; Suzuki, T.; Torii, S.] Waseda Univ, RISE, Tokyo, Japan. [Perrot, A. -L.] CERN, CH-1211 Geneva 23, Switzerland. [Tamura, T.] Kanagawa Univ, Yokohama, Kanagawa, Japan. [Noda, K.; Tricomi, A.] Ist Nazl Fis Nucl, Sect Catania, Catania, Italy. [Tricomi, A.] Univ Catania, I-95124 Catania, Italy. [Turner, W. C.] LBNL, Berkeley, CA USA. RP Sako, T (reprint author), Nagoya Univ, Solar Terr Environm Lab, Nagoya, Aichi 4648601, Japan. EM sako@stelab.nagoya-u.ac.jp RI D'Alessandro, Raffaello/F-5897-2015; Bongi, Massimo/L-9417-2015 OI D'Alessandro, Raffaello/0000-0001-7997-0306; Bongi, Massimo/0000-0002-6050-1937 FU MEXT of Japan; Mitsubishi Foundation in Japan; INFN in Italy; JSPS; INFN; GCOE Program of Nagoya University "QFPU" from JSPS; GCOE Program of Nagoya University "QFPU" from MEXT of Japan FX We thank the CERN staff and the ATLAS collaboration for their essential contributions to the successful operation of LHCf. This work was partly supported by Grant-in-Aid for Scientific Research by MEXT of Japan, the Mitsubishi Foundation in Japan and INFN in Italy. The receipts of a JSPS Research Fellowship (HM), INFN fellowships for non-Italian citizens (HM and KN) and the GCOE Program of Nagoya University "QFPU" from JSPS and MEXT of Japan (GM) are also acknowledged. A part of this work was performed using the computer resources provided by the Institute for the Cosmic-Ray Research (ICRR), University of Tokyo. NR 21 TC 4 Z9 4 U1 1 U2 3 PU WORLD SCIENTIFIC PUBL CO PTE LTD PI SINGAPORE PA 5 TOH TUCK LINK, SINGAPORE 596224, SINGAPORE SN 0217-751X EI 1793-656X J9 INT J MOD PHYS A JI Int. J. Mod. Phys. A PD OCT 10 PY 2013 VL 28 IS 25 AR UNSP 1330036 DI 10.1142/S0217751X13300366 PG 26 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA 233FX UT WOS:000325554200003 ER PT J AU Baldauf, T Seljak, U Smith, RE Hamaus, N Desjacques, V AF Baldauf, Tobias Seljak, Uros Smith, Robert E. Hamaus, Nico Desjacques, Vincent TI Halo stochasticity from exclusion and nonlinear clustering SO PHYSICAL REVIEW D LA English DT Article ID LARGE-SCALE STRUCTURE; DARK-MATTER HALOES; OCCUPATION DISTRIBUTION; PERTURBATION-THEORY; ANALYTIC MODEL; GALAXIES; PEAKS; STATISTICS; MASS; SIMULATIONS AB The clustering of galaxies in ongoing and upcoming galaxy surveys contains a wealth of cosmological information, but extracting this information is a nontrivial task since galaxies and their host haloes are stochastic tracers of the nonlinear matter density field. This stochasticity is usually modeled as the Poisson shot noise, which is constant as a function of wave number with amplitude given by 1/(n) over bar, where (n) over bar is the number density of galaxies. Here we use dark matter haloes in N-body simulations to show evidence for deviations from this simple behavior and develop models that explain the behavior of the stochasticity on large scales. First, haloes are extended, nonoverlapping objects, i.e., their correlation function needs to go to -1 on small scales. This leads to a negative correction to the stochasticity relative to the Poisson value at low wave number k, decreasing to zero for wave numbers large compared to the inverse exclusion scale. Second, haloes show a nonlinear enhancement of clustering outside the exclusion scale, leading to a positive stochasticity correction. Both of these effects go to zero for high k, making the stochasticity scale dependent even for k < 0.1h Mpc(-1). We show that the corrections in the low-k regime are the same in Eulerian and Lagrangian space, but that the transition scale is pushed to smaller scales for haloes observed at present time (Eulerian space), relative to the initial conditions (Lagrangian space). These corrections vary with halo mass, and we present approximate scalings with halo mass and redshift. We also discuss simple applications of these effects to galaxy samples with nonvanishing satellite fraction, where the stochasticity can again deviate strongly from the fiducial Poisson expectation. Overall, these effects affect the clustering of galaxies at a level of a few percent even on very large scales and need to be modeled properly if we want to extract high precision cosmological information from the upcoming galaxy redshift surveys. C1 [Baldauf, Tobias; Seljak, Uros] Univ Zurich, Inst Theoret Phys, CH-8057 Zurich, Switzerland. [Seljak, Uros] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Seljak, Uros] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Seljak, Uros] Ewha Womans Univ, Inst Early Universe, Seoul 120750, South Korea. [Smith, Robert E.] Max Planck Inst Astrophys, D-85748 Garching, Germany. [Hamaus, Nico] Univ Paris 06, Inst Astrophys Paris, F-75014 Paris, France. [Hamaus, Nico] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Desjacques, Vincent] Univ Geneva, Dept Phys Theor, CH-1211 Geneva, Switzerland. [Desjacques, Vincent] Univ Geneva, Ctr Astroparticle Phys, CH-1211 Geneva, Switzerland. RP Baldauf, T (reprint author), Univ Zurich, Inst Theoret Phys, CH-8057 Zurich, Switzerland. EM baldauf@physik.uzh.ch RI Desjacques, Vincent/A-1892-2014 FU NASA ATP [NNX12AG71G]; Swiss National Foundation (SNF) [200021-116696/1]; WCU [R32-10130]; National Science Foundation [1066293]; ERC [246797]; European Research Council; Swiss National Sciences Foundation FX The authors would like to thank Niayesh Afshordi, Kwan Chuen Chan, Donghui Jeong, Patrick McDonald, Teppei Okumura, Fabian Schmidt, Ravi Sheth, Zvonimir Vlah, and Jaiyul Yoo for useful discussions. The simulations were carried out on the ZBOX3 supercomputer at the Institute for Theoretical Physics of the University of Zurich. This work is supported in part by NASA ATP Grant No. NNX12AG71G, Swiss National Foundation (SNF) under Contract No. 200021-116696/1, WCU Grant No. R32-10130, National Science Foundation Grant No. 1066293. T. B. acknowledges the hospitality of the Aspen Center for Physics. R. E. S. acknowledges support from the ERC under advanced Grant No. 246797, "GALFORMOD,'' from the European Research Council. V. D. acknowledges support from the Swiss National Sciences Foundation. NR 52 TC 39 Z9 39 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD OCT 10 PY 2013 VL 88 IS 8 AR 083507 DI 10.1103/PhysRevD.88.083507 PG 24 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 239QK UT WOS:000326040300002 ER PT J AU Cai, YF Chang, YC Chen, PS Easson, DA Qiu, T AF Cai, Yi-Fu Chang, Yu-Chiao Chen, Pisin Easson, Damien A. Qiu, Taotao TI Planck constraints on Higgs modulated reheating of renormalization group improved inflation SO PHYSICAL REVIEW D LA English DT Article ID QUANTUM-GRAVITY; STANDARD MODEL; PHASE-TRANSITION; PERTURBATIONS; UNIVERSE; COSMOLOGY; SCENARIO; FLATNESS; HORIZON AB Within the framework of renormalization group improved inflationary cosmology motivated by asymptotically safe gravity, we study the dynamics of a scalar field which can be interpreted as the Higgs field. The background trajectories of this model can provide sufficient inflationary e-folds and a graceful exit to a radiation dominated phase. We study the possibility of generating primordial curvature perturbations through the Standard Model Higgs boson. This can be achieved under finely tuned parameter choices by making use of the modulated reheating mechanism. The primordial non-Gaussianity is expected to be sizable in this model. Though tightly constrained by the newly released Planck cosmic microwave background data, this model provides a potentially interesting connection between collider and early Universe physics. C1 [Cai, Yi-Fu] McGill Univ, Dept Phys, Montreal, PQ H3A 2T8, Canada. [Chang, Yu-Chiao; Chen, Pisin; Qiu, Taotao] Natl Taiwan Univ, Dept Phys, Taipei 10617, Taiwan. [Chang, Yu-Chiao; Chen, Pisin; Qiu, Taotao] Natl Taiwan Univ, Leung Ctr Cosmol & Particle Astrophys, Taipei 10617, Taiwan. [Chen, Pisin] Natl Taiwan Univ, Grad Inst Astrophys, Taipei 10617, Taiwan. [Chen, Pisin] Stanford Univ, SLAC, Kavli Inst Particle Astrophys & Cosmol, Stanford, CA 94305 USA. [Easson, Damien A.] Arizona State Univ, Dept Phys, Tempe, AZ 85287 USA. RP Cai, YF (reprint author), McGill Univ, Dept Phys, 3600 Univ St, Montreal, PQ H3A 2T8, Canada. EM yifucai@physics.mcgill.ca; f95222075@ntu.edu.tw; chen@slac.stanford.edu; easson@asu.edu; qiutt@ntu.edu.tw RI Cai, Yi-Fu/M-8162-2013 OI Cai, Yi-Fu/0000-0003-0706-8465 FU Department of Physics in McGill University; Taiwan National Science Council [NSC 101-2923-M-002-006-MY3, 101-2628-M-002-006-MY3]; Taiwan National Center for Theoretical Sciences (NCTS); U.S. Department of Energy [DE- AC03-76SF00515]; Cosmology Initiative at ASU; DOE [DE-SC0008016] FX It is a pleasure to thank Robert Brandenberger, Keisuke Izumi, Andrea De Simone, Antonio Riotto, Teruaki Suyama, and Yi Wang for useful discussion and comments on the manuscript. The work of Y.-F.C. is supported in part by Department of Physics in McGill University. Y.-C.C., P. C., and T. Q. are supported by Taiwan National Science Council under Projects No. NSC 101-2923-M-002-006-MY3 and No. 101-2628-M-002-006-MY3 and by Taiwan National Center for Theoretical Sciences (NCTS). P. C. is in addition supported by the U.S. Department of Energy under Contract No. DE- AC03-76SF00515. D. A. E. is supported in part by the Cosmology Initiative at ASU and by DOE Grant No. DE-SC0008016. Y.F.C. is very grateful to P. C. and T. Q. for their hospitality during his visit to the Leung Center for Cosmology and Particle Astrophysics at National Taiwan University while this work was initiated. NR 63 TC 10 Z9 10 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD OCT 10 PY 2013 VL 88 IS 8 AR 083508 DI 10.1103/PhysRevD.88.083508 PG 13 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 239QK UT WOS:000326040300003 ER PT J AU Martin, BA Kalata, W Shaffer, N Fischer, P Luciano, M Loth, F AF Martin, Bryn A. Kalata, Wojciech Shaffer, Nicholas Fischer, Paul Luciano, Mark Loth, Francis TI Hydrodynamic and Longitudinal Impedance Analysis of Cerebrospinal Fluid Dynamics at the Craniovertebral Junction in Type I Chiari Malformation SO PLOS ONE LA English DT Article ID COMPUTATIONAL FLOW-ANALYSIS; FORAMEN MAGNUM; CSF FLOW; CRANIOCERVICAL DECOMPRESSION; MORPHOMETRIC-ANALYSIS; SYMPTOMATIC PATIENTS; OUTFLOW RESISTANCE; VEIN GRAFTS; MR; CHILDREN AB Elevated or reduced velocity of cerebrospinal fluid (CSF) at the craniovertebral junction (CVJ) has been associated with type I Chiari malformation (CMI). Thus, quantification of hydrodynamic parameters that describe the CSF dynamics could help assess disease severity and surgical outcome. In this study, we describe the methodology to quantify CSF hydrodynamic parameters near the CVJ and upper cervical spine utilizing subject-specific computational fluid dynamics (CFD) simulations based on in vivo MRI measurements of flow and geometry. Hydrodynamic parameters were computed for a healthy subject and two CMI patients both pre- and post-decompression surgery to determine the differences between cases. For the first time, we present the methods to quantify longitudinal impedance (LI) to CSF motion, a subject-specific hydrodynamic parameter that may have value to help quantify the CSF flow blockage severity in CMI. In addition, the following hydrodynamic parameters were quantified for each case: maximum velocity in systole and diastole, Reynolds and Womersley number, and peak pressure drop during the CSF cardiac flow cycle. The following geometric parameters were quantified: cross-sectional area and hydraulic diameter of the spinal subarachnoid space (SAS). The mean values of the geometric parameters increased post-surgically for the CMI models, but remained smaller than the healthy volunteer. All hydrodynamic parameters, except pressure drop, decreased post-surgically for the CMI patients, but remained greater than in the healthy case. Peak pressure drop alterations were mixed. To our knowledge this study represents the first subject-specific CFD simulation of CMI decompression surgery and quantification of LI in the CSF space. Further study in a larger patient and control group is needed to determine if the presented geometric and/or hydrodynamic parameters are helpful for surgical planning. C1 [Martin, Bryn A.; Shaffer, Nicholas; Loth, Francis] Univ Akron, Conquer Chiari Res Ctr, Akron, OH 44325 USA. [Martin, Bryn A.; Shaffer, Nicholas; Loth, Francis] Univ Akron, Dept Mech Engn, Akron, OH 44325 USA. [Kalata, Wojciech] Spraying Syst Inc, Wheaton, IL USA. [Fischer, Paul] Argonne Natl Lab, Div Math & Comp Sci, Argonne, IL 60439 USA. [Luciano, Mark] Cleveland Clin Fdn, Dept Neurosurg, Cleveland, OH USA. RP Martin, BA (reprint author), Univ Akron, Conquer Chiari Res Ctr, Akron, OH 44325 USA. EM director@chiari-research.org RI Martin, Bryn/N-6640-2016 OI Martin, Bryn/0000-0003-1234-7880 FU Edward and Gayle Labuda Charitable Fund of the Vanguard Charitable Endowment Program; Conquer Chiari; Labuda Family Foundation; American Syringomyelia Alliance Project; National Institutes for Health NINDS R15 Grant [1R15NS071455-01] FX This work was supported by the Edward and Gayle Labuda Charitable Fund of the Vanguard Charitable Endowment Program, Conquer Chiari, the Labuda Family Foundation, the American Syringomyelia Alliance Project, and the National Institutes for Health NINDS R15 Grant No. 1R15NS071455-01. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 34 TC 7 Z9 7 U1 0 U2 7 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD OCT 10 PY 2013 VL 8 IS 10 AR e75335 DI 10.1371/journal.pone.0075335 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 236QM UT WOS:000325814200011 PM 24130704 ER PT J AU Li, SJ Ha, SJ Kim, HJ Galazka, JM Cate, JHD Jin, YS Zhao, HM AF Li, Sijin Ha, Suk-Jin Kim, Hee Jin Galazka, Jonathan M. Cate, Jamie H. D. Jin, Yong-Su Zhao, Huimin TI Investigation of the functional role of aldose 1-epimerase in engineered cellobiose utilization SO JOURNAL OF BIOTECHNOLOGY LA English DT Article DE Cellobiose; beta-Glucosidase; Aldose 1-epimerase; Cellulosic ethanol; Mutarotase ID SACCHAROMYCES-CEREVISIAE; FERMENTATION; DEGRADATION; LACTOSE; FUNGUS; YEAST AB Functional expression of a cellodextrin transporter and an intracellular beta-glucosidase from Neurospora crassa in Saccharomyces cerevisiae enables simultaneous co-fermentation of cellobiose and non-glucose sugars such as xylose. Here we investigate the functional role of aldose 1-epimerase (AEP) in engineered cellobiose utilization. One AEP (Ga110) and two putative AEPs (Yhr210c and Ynr071c sharing 50.6% and 51.0% amino acid identity with Ga110, respectively) were selected. Deletion of GAL10 led to complete loss of both AEP activity and cell growth on cellobiose, while GAL 10 complementation restored the AEP activity and cell growth. In addition, deletion of YHR210C or YNR071C resulted in improved cellobiose utilization. These results suggest that the intracellular mutarotation of beta-glucose to alpha-glucose might be a rate controlling step and Gal 10 play a crucial role in cellobiose fermentation by engineered S. cerevisiae. (C) 2013 Elsevier B.V. All rights reserved. C1 [Li, Sijin; Zhao, Huimin] Univ Illinois, Dept Chem & Biomol Engn, Urbana, IL 61801 USA. [Ha, Suk-Jin; Kim, Hee Jin; Jin, Yong-Su] Univ Illinois, Dept Food Sci & Human Nutr, Urbana, IL 61801 USA. [Galazka, Jonathan M.; Cate, Jamie H. D.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Cate, Jamie H. D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Zhao, Huimin] Univ Illinois, Dept Chem, Urbana, IL 61801 USA. [Zhao, Huimin] Univ Illinois, Dept Biochem, Urbana, IL 61801 USA. [Zhao, Huimin] Univ Illinois, Dept Bioengn, Urbana, IL 61801 USA. EM sijinli1@illinois.edu; hashy@illinois.edu; hkim248@illinois.edu; jgalazka@berkeley.edu; jcate@lbl.gov; ysjin@illinois.edu; zhao5@illinois.edu RI Jin, Yong-Su/L-4530-2013; OI Galazka, Jonathan/0000-0002-4153-0249 FU Energy Biosciences Institute FX This work was supported by funding from the Energy Biosciences Institute to Huimin Zhao and Yong-Su Jin. NR 19 TC 2 Z9 2 U1 1 U2 15 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-1656 EI 1873-4863 J9 J BIOTECHNOL JI J. Biotechnol. PD OCT 10 PY 2013 VL 168 IS 1 BP 1 EP 6 DI 10.1016/j.jbiotec.2013.08.003 PG 6 WC Biotechnology & Applied Microbiology SC Biotechnology & Applied Microbiology GA 232BT UT WOS:000325464300002 PM 23954547 ER PT J AU Dudy, L Denlinger, JD Shu, L Janoschek, M Allen, JW Maple, MB AF Dudy, L. Denlinger, J. D. Shu, L. Janoschek, M. Allen, J. W. Maple, M. B. TI Yb valence change in Ce1-xYbxCoIn5 from spectroscopy and bulk properties SO PHYSICAL REVIEW B LA English DT Article ID KONDO-LATTICE; SUPERCONDUCTING PHASES; FERMI-SURFACE; CECOIN5; PHOTOEMISSION; TRANSITIONS; SCATTERING; PRESSURE; METALS; STATES AB The electronic structure of Ce1-xYbxCoIn5 has been studied by a combination of photoemission, x-ray absorption, and bulk property measurements. Previous findings of a Ce valence near 3+ for all x and of an Yb valence near 2.3+ for x >= 0.3 were confirmed. One new result of this study is that the Yb valence for x <= 0.2 increases rapidly with decreasing x from 2.3 toward 3+, which correlates well with de Haas van Alphen results showing a change of Fermi surface around x = 0.2. Another new result is the direct observation by angle resolved photoemission Fermi surface maps of approximate to 50% cross-sectional area reductions of the alpha and beta sheets for x = 1 compared to x = 0, and a smaller, essentially proportionate, size change of the a sheet for x = 0.2. These changes are found to be in good general agreement with expectations from simple electron counting. The implications of these results for the unusual robustness of superconductivity and Kondo coherence with increasing x in this alloy system are discussed. C1 [Dudy, L.; Allen, J. W.] Univ Michigan, Randall Lab, Ann Arbor, MI 48109 USA. [Dudy, L.] Univ Wurzburg, Inst Phys, D-97074 Wurzburg, Germany. [Dudy, L.] Univ Wurzburg, Rontgen Ctr Complex Mat Syst, D-97074 Wurzburg, Germany. [Denlinger, J. D.] Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94270 USA. [Shu, L.; Janoschek, M.; Maple, M. B.] Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. [Shu, L.] Fudan Univ, Dept Phys, State Key Lab Surface Phys, Shanghai 200433, Peoples R China. [Janoschek, M.] Los Alamos Natl Lab, Condensed Matter & Magnet Sci Grp, Los Alamos, NM 87545 USA. RP Dudy, L (reprint author), Univ Michigan, Randall Lab, Ann Arbor, MI 48109 USA. RI Janoschek, Marc/M-8871-2015 OI Janoschek, Marc/0000-0002-2943-0173 FU US DOE at the ALS [DE-AC02-05CH11231]; US DOE at UM [DE-FG02-07ER46379]; US DOE at UCSD [DE FG02-04ER-46105]; US NSF at UM [DMR-03-02825]; NSF [DMR-0320740]; Alexander von Humboldt foundation FX This work was supported by the US DOE at the ALS, Contract No. DE-AC02-05CH11231, at UM, Contract No. DE-FG02-07ER46379 for current work, and at UCSD, Contract No. DE FG02-04ER-46105; by the US NSF at UM, Grant No. DMR-03-02825 for initial work. The experimental support at ALS beamline 7.0 by E. Rotenberg is gratefully acknowledged. For the EDX measured at the EMAL at the UM, we thank J. Mansfield for discussion and acknowledge the support of NSF grant DMR-0320740. M.J. acknowledges support by the Alexander von Humboldt foundation. We thank Sooyoung Jang for assistance in the preparation of Fig. 7. NR 49 TC 14 Z9 14 U1 2 U2 32 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 10 PY 2013 VL 88 IS 16 AR 165118 DI 10.1103/PhysRevB.88.165118 PG 14 WC Physics, Condensed Matter SC Physics GA 232OQ UT WOS:000325503800002 ER PT J AU Knut, R Svedlindh, P Mryasov, O Gunnarsson, K Warnicke, P Arena, DA Bjorck, M Dennison, AJC Sahoo, A Mukherjee, S Sarma, DD Granroth, S Gorgoi, M Karis, O AF Knut, Ronny Svedlindh, Peter Mryasov, Oleg Gunnarsson, Klas Warnicke, Peter Arena, D. A. Bjoerck, Matts Dennison, Andrew J. C. Sahoo, Anindita Mukherjee, Sumanta Sarma, D. D. Granroth, Sari Gorgoi, Mihaela Karis, Olof TI Interface characterization of Co2MnGe/Rh2CuSn Heusler multilayers SO PHYSICAL REVIEW B LA English DT Article ID HALF-METALLIC FERROMAGNETS; RAY CIRCULAR-DICHROISM; BAND-STRUCTURE; MAGNETORESISTANCE; DISORDER; ELEMENTS AB To address the amount of disorder and interface diffusion induced by annealing, all-Heusler multilayer structures, consisting of ferromagnetic Co2MnGe and nonmagnetic Rh2CuSn layers of varying thicknesses, have been investigated by means of hard x-ray photoelectron spectroscopy and x-ray magnetic circular dichroism. We find evidence for a 4 angstrom thick magnetically dead layer that, together with the identified interlayer diffusion, are likely reasons for the unexpectedly small magnetoresistance found for current-perpendicular-to-plane giant magnetoresistance devices based on this all-Heusler system. We find that diffusion begins already at comparably low temperatures between 200 and 250 degrees C, where Mn appears to be most prone to diffusion. C1 [Knut, Ronny; Bjoerck, Matts; Dennison, Andrew J. C.; Sarma, D. D.; Karis, Olof] Uppsala Univ, Dept Phys & Astron, S-75120 Uppsala, Sweden. [Svedlindh, Peter; Gunnarsson, Klas] Uppsala Univ, Dept Engn Sci, S-75121 Uppsala, Sweden. [Mryasov, Oleg] Univ Alabama, Dept Phys & Astron, Tuscaloosa, AL 35487 USA. [Mryasov, Oleg] Univ Alabama, MINT Ctr, Tuscaloosa, AL 35487 USA. [Warnicke, Peter; Arena, D. A.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Dennison, Andrew J. C.] Inst Laue Langevin, F-38042 Grenoble, France. [Sahoo, Anindita] Indian Inst Sci, Dept Phys, Bangalore 560012, Karnataka, India. [Sahoo, Anindita; Mukherjee, Sumanta; Sarma, D. D.] Indian Inst Sci, Solid State & Struct Chem Unit, Bangalore 560012, Karnataka, India. [Granroth, Sari] Univ Turku, Dept Phys, Turku, Finland. [Gorgoi, Mihaela] Helmholtz Zentrum Berlin Mat & Energie GmbH, BESSY 2, Berlin, Germany. RP Knut, R (reprint author), Uppsala Univ, Dept Phys & Astron, Box 516, S-75120 Uppsala, Sweden. RI Svedlindh, Peter/K-2702-2012; Gorgoi, Mihaela/N-8831-2014; OI Karis, Olof/0000-0001-6406-217X; Warnicke, Peter/0000-0002-5252-6392 FU Swedish Research Council (VR); Swedish Foundation for International Cooperation in Research and Higher Education (STINT); SuperAdam; European Community [226716]; Goran Gustavsson Foundation FX This work was supported by the Swedish Research Council (VR) and the Swedish Foundation for International Cooperation in Research and Higher Education (STINT). VR is also acknowledged for their financial support of SuperAdam. We acknowledge the Helmholtz-Zentrum Berlin-Electron storage ring BESSY II for provision of synchrotron radiation at beamline KMC-1. We also would like to thank M. Mertin for assistance. The research leading to these results has received funding from the European Community's Seventh Framework Programme (FP7/2007-2013) under Grant Agreement No. 226716. O.K. gratefully acknowledges the support of the Goran Gustavsson Foundation. NR 36 TC 4 Z9 4 U1 1 U2 37 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 10 PY 2013 VL 88 IS 13 AR 134407 DI 10.1103/PhysRevB.88.134407 PG 8 WC Physics, Condensed Matter SC Physics GA 232MI UT WOS:000325497600001 ER PT J AU Lee, CH Kim, JH Zou, CY Cho, IS Weisse, JM Nemeth, W Wang, Q Van Duin, ACT Kim, TS Zheng, XL AF Lee, Chi Hwan Kim, Jae-Han Zou, Chenyu Cho, In Sun Weisse, Jeffery M. Nemeth, William Wang, Qi Van Duin, Adri C. T. Kim, Taek-Soo Zheng, Xiaolin TI Peel-and-Stick: Mechanism Study for Efficient Fabrication of Flexible/Transparent Thin-film Electronics SO SCIENTIFIC REPORTS LA English DT Article ID REACTIVE FORCE-FIELD; ADHESION; REAXFF; ENERGY AB Peel-and-stick process, or water-assisted transfer printing (WTP), represents an emerging process for transferring fully fabricated thin-film electronic devices with high yield and fidelity from a SiO2/Si wafer to various non-Si based substrates, including papers, plastics and polymers. This study illustrates that the fundamental working principle of the peel-and-stick process is based on the water-assisted subcritical debonding, for which water reduces the critical adhesion energy of metal-SiO2 interface by 70 similar to 80%, leading to clean and high quality transfer of thin-film electronic devices. Water-assisted subcritical debonding is applicable for a range of metal-SiO2 interfaces, enabling the peel-and-stick process as a general and tunable method for fabricating flexible/transparent thin-film electronic devices. C1 [Lee, Chi Hwan; Cho, In Sun; Weisse, Jeffery M.; Zheng, Xiaolin] Stanford Univ, Dept Mech Engn, Stanford, CA 94305 USA. [Kim, Jae-Han; Kim, Taek-Soo] Korea Adv Inst Sci & Technol, Dept Mech Engn, Taejon 305701, South Korea. [Zou, Chenyu; Van Duin, Adri C. T.] Penn State Univ, Dept Mech & Nucl Engn, University Pk, PA 16802 USA. [Nemeth, William; Wang, Qi] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Zheng, XL (reprint author), Stanford Univ, Dept Mech Engn, Stanford, CA 94305 USA. EM tskim1@kaist.ac.kr; xlzheng@stanford.edu RI Kim, Taek-Soo/C-1843-2011; OI Cho, In Sun/0000-0001-5622-7712 FU Samsung Global Research Outreach Program (SPO) [107915]; National Research Foundation of Korea [NRF-2012R1A1A1006072]; U.S. Department of Energy [DE-AC36-08-GO28308]; National Energy Technology Laboratory-Regional University Association (NETL/RUA) FX X.L.Z. acknowledges the financial support by the Samsung Global Research Outreach Program (SPO#: 107915). T.S.K. acknowledges financial support from the National Research Foundation of Korea (NRF-2012R1A1A1006072). NREL work is supported by the U.S. Department of Energy under contract DE-AC36-08-GO28308. ACTvD and CZ acknowledge funding from the National Energy Technology Laboratory-Regional University Association (NETL/RUA). RES Activity Number 600.220.001 AETRI. NR 29 TC 14 Z9 14 U1 5 U2 64 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD OCT 10 PY 2013 VL 3 AR 2917 DI 10.1038/srep02917 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 232DH UT WOS:000325469500004 PM 24108063 ER PT J AU Li, GR Li, Q Pan, MH Hu, B Chen, C Teng, J Diao, ZY Zhang, JD Jin, RY Plummer, EW AF Li, Guorong Li, Qing Pan, Minghu Hu, Biao Chen, Chen Teng, Jing Diao, Zhenyu Zhang, Jiandi Jin, Rongying Plummer, E. W. TI Atomic-Scale Fingerprint of Mn Dopant at the Surface of Sr-3(Ru1-xMnx)(2)O-7 SO SCIENTIFIC REPORTS LA English DT Article ID SCANNING TUNNELING MICROSCOPE; INSULATOR-TRANSITION; METAL AB Chemical doping in materials is known to give rise to emergent phenomena. These phenomena are extremely difficult to predict a priori, because electron-electron interactions are entangled with local environment of assembled atoms. Scanning tunneling microscopy and low energy electron diffraction are combined to investigate how the local electronic structure is correlated with lattice distortion on the surface of Sr-3(Ru1-xMnx)(2)O-7, which has double-layer building blocks formed by (Ru/Mn)O-6 octahedra with rotational distortion. The presence of doping-dependent tilt distortion of (Ru/Mn)O-6 octahedra at the surface results in a C-2v broken symmetry in contrast with the bulk C-4v counterpart. It also enables us to observe two Mn sites associated with the octahedral rotation in the bulk through the "chirality" of local electronic density of states surrounding Mn, which is randomly distributed. These results serve as fingerprint of chemical doping on the atomic scale. C1 [Li, Guorong; Hu, Biao; Chen, Chen; Teng, Jing; Diao, Zhenyu; Zhang, Jiandi; Jin, Rongying; Plummer, E. W.] Louisiana State Univ, Dept Phys & Astron, Baton Rouge, LA 70803 USA. [Li, Qing; Pan, Minghu] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Li, Qing] Soochow Univ, Inst Funct Nano & Soft Mat FUNSOM, Suzhou 215123, Jiangsu, Peoples R China. RP Plummer, EW (reprint author), Louisiana State Univ, Dept Phys & Astron, Baton Rouge, LA 70803 USA. EM wplummer@phys.lsu.edu RI Li, Guorong/C-3806-2015 FU NSF [DMR-1002622, DMR-1005562]; Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX Research at LSU is supported by NSF DMR-1002622 (GL, RJ, EWP) and NSF DMR-1005562 (JZ). Part of this research was conducted (QL, MP) at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. We would like to thank R. Kurtz for constructive discussions. NR 22 TC 7 Z9 7 U1 0 U2 30 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD OCT 10 PY 2013 VL 3 AR 2882 DI 10.1038/srep02882 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 232DC UT WOS:000325468900001 PM 24108411 ER PT J AU Funsten, HO DeMajistre, R Frisch, PC Heerikhuisen, J Higdon, DM Janzen, P Larsen, BA Livadiotis, G McComas, DJ Mobius, E Reese, CS Reisenfeld, DB Schwadron, NA Zirnstein, EJ AF Funsten, H. O. DeMajistre, R. Frisch, P. C. Heerikhuisen, J. Higdon, D. M. Janzen, P. Larsen, B. A. Livadiotis, G. McComas, D. J. Moebius, E. Reese, C. S. Reisenfeld, D. B. Schwadron, N. A. Zirnstein, E. J. TI CIRCULARITY OF THE INTERSTELLAR BOUNDARY EXPLORER RIBBON OF ENHANCED ENERGETIC NEUTRAL ATOM (ENA) FLUX SO ASTROPHYSICAL JOURNAL LA English DT Article DE ISM: atoms; ISM: kinematics and dynamics; ISM: magnetic fields; ISM: structure; Sun: heliosphere ID IBEX RIBBON; LO OBSERVATIONS; EDGE-DETECTION; HELIOSPHERE; IONS; HELIOSHEATH; HELIOPAUSE; MECHANISM; MODELS; PICKUP AB As a sharp feature in the sky, the ribbon of enhanced energetic neutral atom (ENA) flux observed by the Interstellar Boundary Explorer (IBEX) mission is a key signature for understanding the interaction of the heliosphere and the interstellar medium through which we are moving. Over five nominal IBEX energy passbands (0.7, 1.1, 1.7, 2.7, and 4.3 keV), the ribbon is extraordinarily circular, with a peak location centered at ecliptic (lambda(RC), beta(RC)) = (219 degrees.2 +/- 1 degrees.3, 39 degrees.9 +/- 2 degrees.3) and a half cone angle of phi(C) = 74 degrees.5 +/- 2 degrees.0. A slight elongation of the ribbon, generally perpendicular to the ribbon center-heliospheric nose vector and with eccentricity similar to 0.3, is observed over all energies. At 4.3 keV, the ribbon is slightly larger and displaced relative to lower energies. For all ENA energies, a slice of the ribbon flux peak perpendicular to the circular arc is asymmetric and systematically skewed toward the ribbon center. We derive a spatial coherence parameter delta(C) <= 0.014 that characterizes the spatial uniformity of the ribbon over its extent in the sky and is a key constraint for understanding the underlying processes and structure governing the ribbon ENA emission. C1 [Funsten, H. O.; Higdon, D. M.; Larsen, B. A.; Moebius, E.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [DeMajistre, R.] Johns Hopkins Univ, Appl Phys Lab, Laurel, MD 20723 USA. [Frisch, P. C.] Univ Chicago, Dept Astron & Astrophys, Chicago, IL 60637 USA. [Heerikhuisen, J.; Zirnstein, E. J.] Univ Alabama, Dept Phys, Huntsville, AL 35899 USA. [Heerikhuisen, J.; Zirnstein, E. J.] Univ Alabama, Ctr Space Phys & Aeron Res, Huntsville, AL 35899 USA. [Janzen, P.; Reisenfeld, D. B.] Univ Montana, Missoula, MT 59812 USA. [Livadiotis, G.; McComas, D. J.] SW Res Inst, San Antonio, TX 78228 USA. [McComas, D. J.] Univ Texas San Antonio, Dept Phys & Astron, San Antonio, TX 78249 USA. [Moebius, E.; Schwadron, N. A.] Univ New Hampshire, Durham, NH 03824 USA. [Reese, C. S.] Brigham Young Univ, Dept Stat, Provo, UT 84602 USA. RP Funsten, HO (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM hfunsten@lanl.gov; Bob.DeMajistre@jhuapl.edu; frisch@oddjob.uchicago.edu; jacob.heerikhuisen@uah.edu; dhigdon@lanl.gov; paul.janzen@umontana.edu; balarsen@lanl.gov; george.livadiotis@swri.org; dmccomas@swri.edu; eberhard.moebius@unh.edu; reese@stat.byu.edu; dan.reisenfeld@umontana.edu; nschwadron@unh.edu; Eric.Zirnstein@uah.edu RI Funsten, Herbert/A-5702-2015; Larsen, Brian/A-7822-2011; Reisenfeld, Daniel/F-7614-2015; OI Funsten, Herbert/0000-0002-6817-1039; Larsen, Brian/0000-0003-4515-0208; Moebius, Eberhard/0000-0002-2745-6978; Heerikhuisen, Jacob/0000-0001-7867-3633 FU NASA; US Department of Energy FX We gratefully acknowledge all of the contributions made by the entire IBEX team who have been and continue to make this mission a tremendous success. IBEX and this work were funded by NASA as a part of the Explorer Program. Work at Los Alamos National Laboratory was performed under the auspices of the US Department of Energy. NR 41 TC 44 Z9 44 U1 0 U2 10 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X J9 ASTROPHYS J JI Astrophys. J. PD OCT 10 PY 2013 VL 776 IS 1 AR 30 DI 10.1088/0004-637X/776/1/30 PG 15 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 225UM UT WOS:000324989000030 ER PT J AU Hoffman, J Tung, IC Nelson-Cheeseman, BB Liu, M Freeland, JW Bhattacharya, A AF Hoffman, J. Tung, I. C. Nelson-Cheeseman, B. B. Liu, M. Freeland, J. W. Bhattacharya, A. TI Charge transfer and interfacial magnetism in (LaNiO3)(n)/(LaMnO3)(2) superlattices SO PHYSICAL REVIEW B LA English DT Article ID METAL-INSULATOR-TRANSITION; MIXED-VALENCE MANGANITES; PULSED-LASER DEPOSITION; COLOSSAL MAGNETORESISTANCE; ELECTRONIC-PROPERTIES; THIN-FILMS; HALL; LANIO3; ENHANCEMENT; PEROVSKITES AB (LaNiO3)(n)/(LaMnO3)(2) superlattices were grown using ozone-assisted molecular beam epitaxy, where LaNiO3 is a paramagnetic metal and LaMnO3 is an antiferromagnetic insulator. The superlattices exhibit excellent crystallinity and interfacial roughness of less than one unit cell. X-ray spectroscopy and dichroism measurements indicate that electrons are transferred from the LaMnO3 to the LaNiO3, inducing magnetism in LaNiO3. Magnetotransport measurements reveal a transition from metallic to insulating behavior as the LaNiO3 layer thickness is reduced from five to two unit cells and suggest an inhomogeneous magnetic structure within LaNiO3. C1 [Hoffman, J.; Nelson-Cheeseman, B. B.; Bhattacharya, A.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Tung, I. C.] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. [Tung, I. C.; Freeland, J. W.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Liu, M.; Bhattacharya, A.] Argonne Natl Lab, Nanosci & Technol Div, Argonne, IL 60439 USA. RP Hoffman, J (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM jhoffman@anl.gov; anand@anl.gov RI Bhattacharya, Anand/G-1645-2011; Liu, Ming/B-4143-2009 OI Bhattacharya, Anand/0000-0002-6839-6860; Liu, Ming/0000-0002-6310-948X FU U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX Work at Argonne National Laboratory, including the use of the Center for Nanoscale Materials, supported by the U.S. Department of Energy, Office of Basic Energy Sciences under Contract No. DE-AC02-06CH11357. NR 53 TC 30 Z9 30 U1 2 U2 70 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD OCT 10 PY 2013 VL 88 IS 14 AR 144411 DI 10.1103/PhysRevB.88.144411 PG 7 WC Physics, Condensed Matter SC Physics GA 232NA UT WOS:000325499400005 ER PT J AU Mishra, R Zhou, W Pennycook, SJ Pantelides, ST Idrobo, JC AF Mishra, Rohan Zhou, Wu Pennycook, Stephen J. Pantelides, Sokrates T. Idrobo, Juan-Carlos TI Long-range ferromagnetic ordering in manganese-doped two-dimensional dichalcogenides SO PHYSICAL REVIEW B LA English DT Article ID INITIO MOLECULAR-DYNAMICS; GRAPHENE; TRANSITION; GAAS AB We report an investigation of long-range ferromagnetic (FM) ordering in Mn-doped MoS2, MoSe2, MoTe2, and WS2 for Mn concentration less than 5% using density functional theory calculations. The long-range ferromagnetism of Mn spins is mediated by an antiferromagnetic (AFM) exchange between the localized Mn d states and the delocalized p states of the S, Se, and Te atoms. In contrast, transition metals like Fe, Co, and Ni show a FM exchange with the S, Se, and Te atoms, which results in a very weak FM (even slightly AFM) coupling for transition-metal defects with large separations. The Mn substitution at Mo or W sites is energetically favorable, thus making the Mn-doped dichalcogenides promising candidates for two-dimensional dilute magnetic semiconductors. C1 [Mishra, Rohan; Pantelides, Sokrates T.] Vanderbilt Univ, Dept Phys & Astron, Nashville, TN 37235 USA. [Mishra, Rohan; Zhou, Wu; Pennycook, Stephen J.; Pantelides, Sokrates T.; Idrobo, Juan-Carlos] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Mishra, R (reprint author), Vanderbilt Univ, Dept Phys & Astron, Nashville, TN 37235 USA. EM rohan.mishra@vanderbilt.edu RI Mishra, Rohan/J-9127-2013; Zhou, Wu/D-8526-2011; Idrobo, Juan/H-4896-2015 OI Mishra, Rohan/0000-0003-1261-0087; Zhou, Wu/0000-0002-6803-1095; Idrobo, Juan/0000-0001-7483-9034 FU Materials Sciences and Engineering Division, Office of Basic Energy Sciences (BES), US Department of Energy (DOE); Laboratory Directed Research and Development Program of Oak Ridge National Laboratory; Oak Ridge National Laboratory's Shared Research Equipment (ShaRE) User Facility Program; BES US DOE; Office of Science of the US DOE [DE-AC02-05CH11231] FX This research was supported by the Materials Sciences and Engineering Division, Office of Basic Energy Sciences (BES), US Department of Energy (DOE) (R. M., S.J.P., S. T. P.), by a Wigner Fellowship through the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the US DOE (WZ), by Oak Ridge National Laboratory's Shared Research Equipment (ShaRE) User Facility Program (JCI), which is also sponsored by BES US DOE. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the US DOE under Contract No. DE-AC02-05CH11231. NR 27 TC 66 Z9 66 U1 19 U2 184 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD OCT 10 PY 2013 VL 88 IS 14 AR 144409 DI 10.1103/PhysRevB.88.144409 PG 5 WC Physics, Condensed Matter SC Physics GA 232NA UT WOS:000325499400003 ER PT J AU Fu, PC Johnson, SM Carrigan, CR AF Fu, Pengcheng Johnson, Scott M. Carrigan, Charles R. TI An explicitly coupled hydro-geomechanical model for simulating hydraulic fracturing in arbitrary discrete fracture networks SO INTERNATIONAL JOURNAL FOR NUMERICAL AND ANALYTICAL METHODS IN GEOMECHANICS LA English DT Article DE hydraulic fracture; discrete fracture network; explicit coupling; fracture interaction; rock joint; reservoir model ID QUARTER-POINT ELEMENTS; STRESS INTENSITY FACTORS; PROPAGATION; ROCK; DISPLACEMENT; MECHANICS; TOUGHNESS; BRITTLE; JOINTS AB Modeling hydraulic fracturing in the presence of a natural fracture network is a challenging task, owing to the complex interactions between fluid, rock matrix, and rock interfaces, as well as the interactions between propagating fractures and existing natural interfaces. Understanding these complex interactions through numerical modeling is critical to the design of optimum stimulation strategies. In this paper, we present an explicitly integrated, fully coupled discrete-finite element approach for the simulation of hydraulic fracturing in arbitrary fracture networks. The individual physical processes involved in hydraulic fracturing are identified and addressed as separate modules: a finite element approach for geomechanics in the rock matrix, a finite volume approach for resolving hydrodynamics, a geomechanical joint model for interfacial resolution, and an adaptive remeshing module. The model is verified against the Khristianovich-Geertsma-DeKlerk closed-form solution for the propagation of a single hydraulic fracture and validated against laboratory testing results on the interaction between a propagating hydraulic fracture and an existing fracture. Preliminary results of simulating hydraulic fracturing in a natural fracture system consisting of multiple fractures are also presented. Copyright (c) 2012 John Wiley & Sons, Ltd. C1 [Fu, Pengcheng; Johnson, Scott M.; Carrigan, Charles R.] Lawrence Livermore Natl Lab, Atmospher Earth & Energy Div, Livermore, CA 94550 USA. RP Fu, PC (reprint author), Lawrence Livermore Natl Lab, Atmospher Earth & Energy Div, 7000 East Ave,L-286, Livermore, CA 94550 USA. EM fu4@llnl.gov RI Fu, Pengcheng/D-7483-2012 OI Fu, Pengcheng/0000-0002-7408-3350 FU Geothermal Technologies Program of the US Department of Energy under Enhanced Geothermal Systems Program; Lawrence Livermore National Laboratory (LLNL) LDRD project 'Creating Optimal Fracture Networks' [11-SI-006]; US Department of Energy by LLNL [DE-AC52-07NA27344] FX The authors gratefully acknowledge the Geothermal Technologies Program of the US Department of Energy for support of this work under the Enhanced Geothermal Systems Program. Additional support was provided by the Lawrence Livermore National Laboratory (LLNL) LDRD project 'Creating Optimal Fracture Networks' (#11-SI-006). The authors also would like to acknowledge their collaborators at the LLNL. This work was performed under the auspices of the US Department of Energy by LLNL under Contract DE-AC52-07NA27344. This paper is LLNL Report LLNL-JRNL-519272. NR 46 TC 42 Z9 46 U1 4 U2 73 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0363-9061 J9 INT J NUMER ANAL MET JI Int. J. Numer. Anal. Methods Geomech. PD OCT 10 PY 2013 VL 37 IS 14 BP 2278 EP 2300 DI 10.1002/nag.2135 PG 23 WC Engineering, Geological; Materials Science, Multidisciplinary; Mechanics SC Engineering; Materials Science; Mechanics GA 213AS UT WOS:000324025900009 ER PT J AU Zhao, YC Huang, CS Kim, M Wong, BM Leonard, F Gopalan, P Eriksson, MA AF Zhao, Yuanchun Huang, Changshui Kim, Myungwoong Wong, Bryan M. Leonard, Francois Gopalan, Padma Eriksson, Mark A. TI Functionalization of Single-Wall Carbon Nanotubes with Chromophores of Opposite Internal Dipole Orientation SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE functionalization; single-wall carbon nanotube; chromophore; dipole orientation; field-effect transistor; DFT calculations ID FIELD-EFFECT TRANSISTORS; CHARGE-TRANSFER; MOLECULES; CHEMISTRY; DEVICES; SENSORS AB We report the functionalization of carbon nanotubes with two azobenzene-based chromophores with large internal dipole moments and opposite dipole orientations. The molecules are attached to the nanotubes noncovalently via a pyrene tether. A combination of characterization techniques shows uniform molecular coverage on the nanotubes, with minimal aggregation of excess chromophores on the substrate. The large on/off ratios and the subthreshold swings of the nanotube-based field-effect transistors (FETs) are preserved after functionalization, and different shifts in threshold voltage are observed for each chromophore. Ab initio calculations verify the properties of the synthesized chromophores and indicate very small charge transfer, confirming a strong, noncovalent functionalization. C1 [Zhao, Yuanchun; Eriksson, Mark A.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Huang, Changshui; Kim, Myungwoong; Gopalan, Padma] Univ Wisconsin, Dept Mat Sci & Engn, Madison, WI 53706 USA. [Wong, Bryan M.; Leonard, Francois] Sandia Natl Labs, Livermore, CA 94551 USA. RP Gopalan, P (reprint author), Univ Wisconsin, Dept Mat Sci & Engn, 1509 Univ Ave, Madison, WI 53706 USA. EM pgopalan@wisc.edu; maeriksson@wisc.edu RI Zhao, Yuanchun/H-8763-2012; Wong, Bryan/B-1663-2009; Huang, Changshui /A-4561-2013 OI Wong, Bryan/0000-0002-3477-8043; FU Division of Materials Sciences and Engineering, Office of Basic Energy Science, U.S. Department of Energy [ER46590]; National Science Foundation [TG-CHE130052] FX We acknowledge financial support from the Division of Materials Sciences and Engineering, Office of Basic Energy Science, U.S. Department of Energy, under Award ER46590. B.M.W. acknowledges the National Science Foundation for supercomputing resources through the Extreme Science and Engineering Discovery Environment (XSEDE), Project TG-CHE130052. NR 38 TC 12 Z9 12 U1 5 U2 41 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 EI 1944-8252 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD OCT 9 PY 2013 VL 5 IS 19 BP 9355 EP 9361 DI 10.1021/am4024753 PG 7 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA 243ZJ UT WOS:000326356600015 PM 24060382 ER PT J AU Wang, H Shen, J Li, YY Wei, ZY Cao, GX Gai, Z Hong, KL Banerjee, P Zhou, SQ AF Wang, Hui Shen, Jing Li, Yingyu Wei, Zengyan Cao, Guixin Gai, Zheng Hong, Kunlun Banerjee, Probal Zhou, Shuiqin TI Porous Carbon Protected Magnetite and Silver Hybrid Nanoparticles: Morphological Control, Recyclable Catalysts, and Multicolor Cell Imaging SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE magnetite-silver hybrid nanoparticles; porous carbon shell; core-satellite and dumbbell-like; catalytic activity; cell imaging ID IRON-OXIDE NANOPARTICLES; ONE-POT SYNTHESIS; BIOMEDICAL APPLICATIONS; GOLD NANOPARTICLES; DRUG-DELIVERY; SHELL NANOPARTICLES; NANOSTRUCTURES; FLUORESCENCE; FABRICATION; NANOCOMPOSITES AB A simple and facile synthetic strategy is developed to prepare a new class of multifunctional hybrid nanoparticles (NPs) that can integrate a magnetic core with silver nanocrystals embedded in porous carbon shell: The method involves a one-step solvothermal synthesis of Fe3O4@C template NPs with Fe(3)O(4)nanocrystals in the core protected by a porous carbon shell, followed by loading and in situ reduction of silver ions in the carbon shell in water at room temperature. The core satellite and dumbbell-like nanostructures of the resulted Fe3O4@C-Ag hybrid NPs can be readily controlled by loading amount of silver ions. The hybrid NPs can efficiently catalyze the reduction reaction of organic dyes in water. The easy magnetic separation and high stability of the catalytically active silver nanocrystals embedded in the carbon shell enable the hybrid NPs to be recycled for reuse as catalysts. The hybrid NPs can also overcome cellular barriers to enter the intracellular region and light up the mouse melanoma B16F10 cells in multicolor modal, with no cytotoxicity. Such porous carbon protected Fe3O4@C-Ag hybrid NPs with controllable nanostructures and a combination of magnetic and noble metallic components have great potential for a broad range of applications in the catalytic industry and biomedical field. C1 [Wang, Hui; Shen, Jing; Li, Yingyu; Banerjee, Probal; Zhou, Shuiqin] CUNY Coll Staten Isl, Dept Chem, Staten Isl, NY 10314 USA. [Wang, Hui; Shen, Jing; Li, Yingyu; Banerjee, Probal; Zhou, Shuiqin] CUNY, Grad Ctr, Staten Isl, NY 10314 USA. [Wei, Zengyan] CUNY Hunter Coll, Dept Chem & Biochem, New York, NY 10065 USA. [Cao, Guixin; Gai, Zheng; Hong, Kunlun] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Zhou, SQ (reprint author), CUNY Coll Staten Isl, Dept Chem, Staten Isl, NY 10314 USA. EM shuiqin.zhou@csi.cuny.edu RI Gai, Zheng/B-5327-2012; Wei, Zengyan/B-1548-2012; wang, hui/G-6433-2015; Cao, Guixin/G-4452-2015; Hong, Kunlun/E-9787-2015 OI Gai, Zheng/0000-0002-6099-4559; Wei, Zengyan/0000-0001-6948-7572; Cao, Guixin/0000-0002-9252-1158; Hong, Kunlun/0000-0002-2852-5111 FU PSC-CUNY [64511-00 42]; American Diabetes Association [1-12-BS-243]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX We gratefully acknowledge the financial support from the PSC-CUNY Research Award (64511-00 42) and American Diabetes Association (Basic Science Award 1-12-BS-243). A portion of this research was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. NR 69 TC 24 Z9 26 U1 8 U2 108 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 EI 1944-8252 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD OCT 9 PY 2013 VL 5 IS 19 BP 9446 EP 9453 DI 10.1021/am4032532 PG 8 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA 243ZJ UT WOS:000326356600028 PM 24001139 ER PT J AU Wu, HC Rogalski, M Kessler, MR AF Wu, Hongchao Rogalski, Mark Kessler, Michael R. TI Zirconium Tungstate/Epoxy Nanocomposites: Effect of Nanoparticle Morphology and Negative Thermal Expansivity SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE negative thermal expansion; zirconium tungstate nanoparticle; polymer-matrix composites (PMCs); thermo-mechanical properties; dielectric properties ID CARBON NANOTUBE/EPOXY COMPOSITES; GLASS-TRANSITION TEMPERATURE; CYANATE ESTER COMPOSITES; MECHANICAL-PROPERTIES; EPOXY NANOCOMPOSITES; DIELECTRIC-PROPERTIES; FUMED SILICA; BEHAVIOR; ZRW2O8; COEFFICIENT AB The ability to tailor the coefficient of thermal expansion (CTE) of a polymer is essential for mitigating thermal residual stress and reducing microcracks caused by CTE mismatch of different components in electronic applications. This work studies the effect of morphology and thermal expansivity of zirconium tungstate nanoparticles on the rheological, thermo-mechanical, dynamic-mechanical, and dielectric properties of ZrW2O8/epoxy nanocomposites. Three types of ZrW2O8 nanoparticles were synthesized under different hydrothermal conditions and their distinct properties were characterized, including morphology, particle size, aspect ratio, surface area, and CTE. Nanoparticles with a smaller particle size and larger surface area led to a more significant reduction in gel-time and glass transition temperature of the epoxy nanocomposites, while a higher initial viscosity and significant shear thinning behavior was found in prepolymer suspensions containing ZrW2O8 with larger particle sizes and aspect ratios. The thermo- and dynamic-mechanical properties of epoxy-based nanocomposites improved with increasing loadings of the three types of ZrW2O8 nanoparticles. In addition, the introduced ZrW2O8 nanoparticles did not negatively affect the dielectric constant or the breakdown strength of the epoxy resin, suggesting potential applications of ZrW2O8/epoxy nanocomposites in the microelectronic insulation industry. C1 [Wu, Hongchao; Rogalski, Mark; Kessler, Michael R.] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. [Kessler, Michael R.] US DOE, Ames Lab, Ames, IA 50011 USA. [Kessler, Michael R.] Washington State Univ, Sch Mech & Mat Engn, Pullman, WA 99164 USA. RP Kessler, MR (reprint author), Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. EM MichaelR.Kessler@wsu.edu RI Kessler, Michael/C-3153-2008; Wu, Hongchao/D-4808-2016 OI Kessler, Michael/0000-0001-8436-3447; Wu, Hongchao/0000-0002-0195-8398 FU Honeywell Federal Manufacturing & Technologies, LLC; Air Force Office of Scientific Research [FA9550-12-1-0108] FX The authors gratefully acknowledge partial funding for this project from Honeywell Federal Manufacturing & Technologies, LLC and the Air Force Office of Scientific Research (Award No. FA9550-12-1-0108). The authors also acknowledge Tracey Pepper (Genetics, Development & Cell Biology, Iowa State University) for her assistance with TEM measurements. NR 53 TC 14 Z9 14 U1 7 U2 65 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 EI 1944-8252 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD OCT 9 PY 2013 VL 5 IS 19 BP 9478 EP 9487 DI 10.1021/am402242g PG 10 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA 243ZJ UT WOS:000326356600032 PM 24070222 ER PT J AU Heberle, FA Doktorova, M Goh, SL Standaert, RF Katsaras, J Feigenson, GW AF Heberle, Frederick A. Doktorova, Milka Goh, Shih Lin Standaert, Robert F. Katsaras, John Feigenson, Gerald W. TI Hybrid and Nonhybrid Lipids Exert Common Effects on Membrane Raft Size and Morphology SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID RESONANCE ENERGY-TRANSFER; BIOLOGICAL-MEMBRANES; MODEL BIOMEMBRANES; MODULATED PHASES; BILAYER MIXTURES; DOMAIN FORMATION; PLASMA-MEMBRANE; CRITICAL-POINTS; LINE TENSION; DSPC/DOPC/POPC/CHOL AB Nanometer-scale domains in cholesterol-rich model membranes emulate lipid rafts in cell plasma membranes (PMs). The physicochemical mechanisms that maintain a finite, small domain size are, however, not well understood. A special role has been postulated for chain-asymmetric or hybrid lipids having a saturated sn-1 chain and an unsaturated sn-2 chain. Hybrid lipids generate nanodomains in some model membranes and are also abundant in the PM. It was proposed that they align in a preferred orientation at the boundary of ordered and disordered phases, lowering the interfacial energy and thus reducing domain size. We used small-angle neutron scattering and fluorescence techniques to detect nanoscopic and modulated liquid phase domains in a mixture composed entirely of nonhybrid lipids and cholesterol. Our results are indistinguishable from those obtained previously for mixtures containing hybrid lipids, conclusively showing that hybrid lipids are not required for the formation of nanoscopic liquid domains and strongly implying a common mechanism for the overall control of raft size and morphology. We discuss implications of these findings for theoretical descriptions of nanodomains. C1 [Heberle, Frederick A.; Standaert, Robert F.; Katsaras, John] Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA. [Standaert, Robert F.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. [Doktorova, Milka; Goh, Shih Lin; Feigenson, Gerald W.] Cornell Univ, Dept Mol Biol & Genet, Ithaca, NY 14853 USA. [Doktorova, Milka] Cornell Univ, Triinst Training Program Computat Biol & Med, Ithaca, NY 14853 USA. [Standaert, Robert F.] Univ Tennessee, Dept Biochem & Mol & Cellular Biol, Knoxville, TN 37996 USA. [Standaert, Robert F.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Standaert, Robert F.; Katsaras, John] Joint Inst Neutron Sci, Oak Ridge, TN 37831 USA. RP Heberle, FA (reprint author), Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA. EM heberlefa@ornl.gov; gwf3@cornell.edu RI Standaert, Robert/D-9467-2013; OI Standaert, Robert/0000-0002-5684-1322; Katsaras, John/0000-0002-8937-4177 FU National Science Foundation (NSF) [MCB 0842839]; Laboratory Directed Research and Development Program of Oak Ridge National Laboratory (ORNL); U.S. Department of Energy (DOE) [DE-AC05-00OR2275]; Scientific User Facilities Division, Office of Basic Energy Sciences; Office of Biological and Environmental Research, DOE; Cornell University; NSF FX We thank Robin Petruzielo for providing supporting data. Support was received from National Science Foundation (NSF) research award MCB 0842839 (to G.W.F.) and from the Laboratory Directed Research and Development Program (to J.K. and R.F.S.) of Oak Ridge National Laboratory (ORNL), managed by UT-Battelle, LLC, for the U.S. Department of Energy (DOE) under contract no. DE-AC05-00OR2275. This work acknowledges support from the Scientific User Facilities Division, Office of Basic Energy Sciences, and the Office of Biological and Environmental Research, DOE, for research conducted at the BioSANS instrument at ORNL's High Flux Isotope Reactor and Center for Structural Molecular Biology. A portion of this research was conducted using the resources of the Cornell Center for Advanced Computing, which receives funding from Cornell University, the NSF, and other leading public agencies, foundations, and corporations. NR 36 TC 28 Z9 28 U1 2 U2 47 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 EI 1520-5126 J9 J AM CHEM SOC JI J. Am. Chem. Soc. 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Zimmermann, S. Zinonos, Z. Ziolkowski, M. Zitoun, R. Zivkovic, L. Zobernig, G. Zoccoli, A. zur Nedden, M. Zutshi, V. Zwalinski, L. CA ATLAS Collaboration TI Measurement of the Azimuthal Angle Dependence of Inclusive Jet Yields in Pb plus Pb Collisions at root s(NN)=2.76 TeV with the ATLAS Detector SO PHYSICAL REVIEW LETTERS LA English DT Article ID TRANSVERSE-MOMENTUM DEPENDENCE; LEAD-LEAD COLLISIONS; ROOT-S-NN=2.76 TEV; NUCLEAR COLLISIONS; ANISOTROPIC FLOW; PLASMA AB Measurements of the variation of inclusive jet suppression as a function of relative azimuthal angle, Delta phi, with respect to the elliptic event plane provide insight into the path-length dependence of jet quenching. ATLAS has measured the Delta phi dependence of jet yields in 0.14 nb(-1) of root s(NN) = 2.76 TeV Pb + Pb collisions at the LHC for jet transverse momenta p(T) > 45 GeV in different collision centrality bins using an underlying event subtraction procedure that accounts for elliptic flow. The variation of the jet yield with Delta phi was characterized by the parameter, nu(jet)(2), and the ratio of out-of-plane (Delta phi similar to pi/2) to in-plane (Delta phi similar to 0) yields. Nonzero nu(jet)(2) values were measured in all centrality bins for p(T) < 160 GeV. The jet yields are observed to vary by as much as 20% between in-plane and out-of-plane directions. C1 [Edson, W.; Ernst, J.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Chan, K.; Gingrich, D. M.; Moore, R. W.; Pinfold, J. L.; Saddique, A.; Sbrizzi, A.; Subramania, Hs.; Vaque, F. Vives] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakir, O.; Ciftci, A. K.; Ciftci, R.; Yildiz, H. Duran; Kuday, S.] Ankara Univ, Dept Phys, TR-06100 Ankara, Turkey. [Yilmaz, M.] Gazi Univ, Dept Phys, Ankara, Turkey. [Sultansoy, S.] TOBB Univ Econ & Technol, Div Phys, Ankara, Turkey. [Cakir, I. Turk] Turkish Atom Energy Commiss, Ankara, Turkey. 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N.; Iakovidis, G.; Karakostas, K.; Karastathis, N.; Leontsinis, S.; Maltezos, S.; Mountricha, E.; Ntekas, K.; Panagiotopoulou, E.; Papadopoulou, Th. D.; Tsipolitis, G.; Vlachos, S.] Natl Tech Univ Athens, Dept Phys, GR-15773 Zografos, Greece. [Abdinov, O.; Khalil-Zada, F.] Azerbaijan Acad Sci, Inst Phys, Baku 370143, Azerbaijan. [Abdallah, J.; Bosman, M.; Armadans, R. Caminal; Casado, M. P.; Cavalli-Sforza, M.; Conidi, M. C.; Demirkoz, B.; Curull, X. Espinal; Francavilla, P.; Giangiobbe, V.; Parra, G. Gonzalez; Grinstein, S.; Rozas, A. Juste; Korolkov, I.; Le Menedeu, E.; Martinez, M.; Mir, L. M.; Berlingen, J. Montejo; Nadal, J.; Pages, A. Pacheco; Aranda, C. Padilla; Bueso, X. Portell; Riu, I.; Rossetti, V.; Rubbo, F.; Succurro, A.; Tsiskaridze, S.] Univ Autonoma Barcelona, Inst Fis Altes Energies, E-08193 Barcelona, Spain. [Abdallah, J.; Bosman, M.; Armadans, R. Caminal; Casado, M. P.; Cavalli-Sforza, M.; Conidi, M. C.; Demirkoz, B.; Curull, X. Espinal; Francavilla, P.; Giangiobbe, V.; Parra, G. Gonzalez; Grinstein, S.; Rozas, A. Juste; Korolkov, I.; Le Menedeu, E.; Martinez, M.; Mir, L. M.; Berlingen, J. Montejo; Nadal, J.; Pages, A. Pacheco; Aranda, C. Padilla; Bueso, X. Portell; Riu, I.; Rossetti, V.; Rubbo, F.; Succurro, A.; Tsiskaridze, S.] Univ Autonoma Barcelona, Dept Fis, E-08193 Barcelona, Spain. [Krstic, J.; Popovic, D. S.; Sijacki, Dj.; Simic, Lj.] Univ Belgrade, Inst Phys, Belgrade, Serbia. [Agatonovic-Jovin, T.; Bozovic-Jelisavcic, I.; Cirkovic, P.; Mamuzic, J.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia. [Buanes, T.; Burgess, T.; Eigen, G.; Kastanas, A.; Liebig, W.; Lipniacka, A.; Rosendahl, P. L.; Sandaker, H.; Sjursen, T. B.; Stugu, B.; Tonoyan, A.; Ugland, M.] Univ Bergen, Dept Phys & Technol, Bergen, Norway. [Bach, A. M.; Barnett, R. M.; Beringer, J.; Biesiada, J.; Brandt, G.; Calafiura, P.; Caminada, L. M.; Cerri, A.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Copic, K.; Dube, S.; Einsweiler, K.; Gaponenko, A.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Hance, M.; Heinemann, B.; Hinchliffe, I.; Hurwitz, M.; Lavrijsen, W.; Leggett, C.; Loscutoff, P.; Madaras, R. J.; Ovcharova, A.; Griso, S. Pagan; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Skinnari, L. A.; Sood, A.; Tibbetts, M. J.; Tsulaia, V.; Vahsen, S.; Varouchas, D.; Virzi, J.; Yu, D. R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Bach, A. M.; Barnett, R. M.; Beringer, J.; Biesiada, J.; Brandt, G.; Calafiura, P.; Caminada, L. M.; Cerri, A.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Copic, K.; Dube, S.; Einsweiler, K.; Gaponenko, A.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Hance, M.; Heinemann, B.; Hinchliffe, I.; Hurwitz, M.; Lavrijsen, W.; Leggett, C.; Loscutoff, P.; Madaras, R. J.; Ovcharova, A.; Griso, S. Pagan; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Skinnari, L. A.; Sood, A.; Tibbetts, M. J.; Tsulaia, V.; Vahsen, S.; Varouchas, D.; Virzi, J.; Yu, D. R.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Aliev, M.; Kuutmann, E. Bergeaas; Giorgi, F. M.; Grancagnolo, S.; Herbert, G. H.; Herrberg-Schubert, R.; Hristova, I.; Kind, O.; Kolanoski, H.; Kwee, R.; Lacker, H.; Leyton, M.; Lohse, T.; Nikiforov, A.; Rieck, P.; Schulz, H.; Wendland, D.; zur Nedden, M.] Humboldt Univ, Dept Phys, Berlin, Germany. [Agustoni, M.; Ancu, L. S.; Beck, H. P.; Borer, C.; Cervelli, A.; Ereditato, A.; Martin, T. Fonseca; Gallo, V.; Haug, S.; Kruker, T.; Marti, L. F.; Schneider, B.; Sciacca, F. G.; Topfel, C.; Weber, M. S.] Univ Bern, Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Agustoni, M.; Ancu, L. S.; Beck, H. P.; Borer, C.; Cervelli, A.; Ereditato, A.; Martin, T. Fonseca; Gallo, V.; Haug, S.; Kruker, T.; Marti, L. F.; Schneider, B.; Sciacca, F. G.; Topfel, C.; Weber, M. S.] Univ Bern, High Energy Phys Lab, Bern, Switzerland. [Allbrooke, B. M. M.; Bella, L. Aperio; Bansil, H. S.; Bracinik, J.; Charlton, D. G.; Chisholm, A. S.; Daniells, A. C.; Hawkes, C. M.; Head, S. J.; Hillier, S. J.; Mahout, G.; Mclaughlan, T.; Mudd, R. D.; Quijada, J. A. Murillo; Newman, P. R.; Nikolopoulos, K.; Palmer, J. D.; Slater, M.; Thomas, J. P.; Thompson, P. D.; Watkins, P. M.; Watson, A. T.; Watson, M. F.; Wilson, J. A.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Arik, E.; Arik, M.; Istin, S.; Ozcan, V. E.] Bogazici Univ, Dept Phys, Istanbul, Turkey. [Cetin, S. A.] Dogus Univ, Dept Phys, Istanbul, Turkey. [Beddall, A. J.; Beddall, A.; Bingul, A.] Gaziantep Univ, Dept Engn Phys, Gaziantep, Turkey. [Bellagamba, L.; Bindi, M.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; Caforio, D.; Corradi, M.; De Castro, S.; Di Sipio, R.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Giacobbe, B.; Grafstrom, P.; Jha, M. K.; Massa, I.; Mengarelli, A.; Monzani, S.; Negrini, M.; Piccinini, M.; Polini, A.; Rinaldi, L.; Romano, M.; Sbarra, C.; Semprini-Cesari, N.; Spighi, R.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Bindi, M.; Caforio, D.; De Castro, S.; Di Sipio, R.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Grafstrom, P.; Massa, I.; Mengarelli, A.; Monzani, S.; Piccinini, M.; Romano, M.; Semprini-Cesari, N.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, Dipartimento Fis & Astron, Bologna, Italy. [Abajyan, T.; Arutinov, D.; Backhaus, M.; Bechtle, P.; Brock, I.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Ehrenfeld, W.; Geich-Gimbel, Ch.; Glatzer, J.; Gonella, L.; Haefner, P.; Havranek, M.; Hellmich, D.; Hillert, S.; Huegging, F.; Janssen, J.; Khoriauli, G.; Koevesarki, P.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Kruger, H.; Lapoire, C.; Lehmacher, M.; Leyko, A. M.; Liebal, J.; Limbach, C.; Loddenkoetter, T.; Mueller, K.; Nanava, G.; Nattermann, T.; Nuncio-Quiroz, A. -E.; Pohl, D.; Psoroulas, S.; Sarrazin, B.; Schaepe, S.; Schmieden, K.; Schultens, M. J.; Schwindt, T.; Scutti, F.; Stillings, J. A.; Therhaag, J.; Tsung, J. -W.; Uchida, K.; Uhlenbrock, M.; Urquijo, P.; Vogel, A.; von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Wong, K. H. Yau; Zimmermann, R.; Zimmermann, S.] Univ Bonn, Inst Phys, Bonn, Germany. [Ahlen, S. P.; Bernard, C.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, Boston, MA 02215 USA. [Aefsky, S.; Amelung, C.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Daya-Ishmukhametova, R. K.; Fitzgerald, E. A.; Gozpinar, S.; Pomeroy, D.; Sciolla, G.; Zambito, S.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Coutinho, Y. Amaral; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio de Janeiro, COPPE EE IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; Filho, L. Manhaes de Andrade] Univ Fed Juiz de Fora, Juiz de Fora, Brazil. [do Vale, M. A. B.] Fed Univ Sao Joao Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadelli, M.; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gadfort, T.; Gibbard, B.; Gordon, H. A.; Hu, X.; Klimentov, A.; Kravchenko, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Metcalfe, J.; Nevski, P.; Okawa, H.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Pleier, M. -A.; Polychronakos, V.; Pravahan, R.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Snyder, S.; Steinberg, P.; Stumer, I.; Takai, H.; Triplett, N.; Undrus, A.; Wenaus, T.; Ye, S.; Zaytsev, A.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Badescu, E.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Cuciuc, C. -M.; Dinut, F.; Dita, P.; Dita, S.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. [Darlea, G. L.] Univ Politehn Bucuresti, Bucharest, Romania. [Popeneciu, G. A.] West Univ Timisoara, Timisoara, Romania. [Silva, M. L. Gonzalez; Otero y Garzon, G.; Piegaia, R.; Romeo, G.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Ask, S.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Buttinger, W.; Carter, J. R.; Chapman, J. D.; French, S. T.; Frost, J. A.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Moeller, V.; Mueller, T.; Parker, M. A.; Robinson, D.; Sandoval, T.; Thomson, M.; Ward, C. P.; Williams, S.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Koffas, T.; Lacey, J.; Marchand, J. F.; McCarthy, T. G.; Oakham, F. G.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Anastopoulos, C.; Andari, N.; Anghinolfi, F.; Avolio, G.; Baak, M. A.; Banfi, D.; Battistin, M.; Bellomo, M.; Beltramello, O.; Berge, D.; Bogaerts, J. A.; Boyd, J.; Bremer, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Catmore, J. R.; Cattai, A.; Barajas, C. A. Chavez; Childers, J. T.; Chromek-Burckhart, D.; Danielsson, H. O.; Dell'Acqua, A.; Dewhurst, A.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dopke, J.; Dudarev, A.; Duhrssen, M.; Ellis, N.; Elsing, M.; Fabre, C.; Facini, G.; Farthouat, P.; Fassnacht, P.; Franchino, S.; Francis, D.; Froidevaux, D.; Gabaldon, C.; Garonne, V.; Gianotti, F.; Gillberg, D.; Godlewski, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Haas, S.; Hauschild, M.; Hawkings, R. J.; Heller, M.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Hubacek, Z.; Huhtinen, M.; Jaekel, M. R.; Jansen, H.; Jenni, P.; Jungst, R. M.; Kaneda, M.; Klioutchnikova, T.; Lantzsch, K.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mapelli, L.; Martin, B.; Messina, A.; Meyer, J.; Michal, S.; Molfetas, A.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Negri, G.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Ohm, C. C.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Petersen, J.; Pommes, K.; Poppleton, A.; Poulard, G.; Prasad, S.; Raymond, M.; Rembser, C.; Dos Santos, D. Roda; Roe, S.; Salek, D.; Salzburger, A.; Savu, D. O.; Schlenker, S.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Spiwoks, R.; Stewart, G. A.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van der Ster, D.; van Eldik, N.; Vandelli, W.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. 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[Han, L.; Jiang, Y.; Li, B.; Li, S.; Liu, J. B.; Liu, K.; Liu, M.; Liu, Y.; Peng, H.; Xu, C.; Xu, L.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Yang, H.] Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200030, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] CNRS, IN2P3, Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Chen, Y.; Cole, B.; Dodd, J.; Guo, J.; Hu, D.; Hughes, E. W.; Nikiforou, N.; Parsons, J. A.; Penson, A.; Perepelitsa, D. V.; Reale, V. Perez; Scherzer, M. I.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Williams, E.; Willis, W.; Wulf, E.; Zivkovic, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Boelaert, N.; Dam, M.; Galster, G.; Gregersen, K.; Hansen, J. R.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Heisterkamp, S.; Jakobsen, S.; Joergensen, M. D.; Kadlecik, P.; Klinkby, E. B.; Loevschall-Jensen, A. E.; Mackeprang, R.; Mehlhase, S.; Monk, J.; Petersen, T. C.; Pingel, A.; Simonyan, M.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, DK-2100 Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Grp Coll Cosenza, Cosenza, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartmento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; Blocki, J.; de Renstrom, P. A. Bruckman; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Malecki, P.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Turala, M.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.; Zemla, A.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Cao, T.; Yagci, K. Dindar; Firan, A.; Hoffman, J.; Joffe, D.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Rios, R. R.; Sekula, S. J.; Stroynowski, R.; Wang, H.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Ahsan, M.; Izen, J. M.; Lou, X.; Namasivayam, H.; Reeves, K.; Wong, W. C.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Dassoulas, J. A.; Dietrich, J.; Ferrara, V.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Goebel, M.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Hiller, K. H.; Huettmann, A.; Belenguer, M. Jimenez; Johnert, S.; Katzy, J.; Kono, T.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Cavalcanti, T. Perez; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.; Zhu, H.] DESY, Hamburg, Germany. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Dassoulas, J. A.; Dietrich, J.; Ferrara, V.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Goebel, M.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Hiller, K. H.; Huettmann, A.; Belenguer, M. Jimenez; Johnert, S.; Katzy, J.; Kono, T.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Cavalcanti, T. Perez; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.; Zhu, H.] DESY, Zeuthen, Germany. [Bunse, M.; Esch, H.; Gossling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Reisinger, I.; Wittig, T.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Czodrowski, P.; Friedrich, F.; Grohs, J. P.; Kobel, M.; Leonhardt, K.; Mader, W. F.; Morgenstern, M.; Prudent, X.; Rudolph, C.; Schnoor, U.; Seifert, F.; Steinbach, P.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B.; Finelli, K. D.; Ko, B. R.; Kotwal, A.; Kruse, M. K.; Liu, M.; Oh, S. H.; Pollard, C. S.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Buckley, A. G.; Clark, P. J.; Debenedetti, C.; Walls, F. M. Garay; Harrington, R. D.; Korn, A.; Martin, V. J.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Schaelicke, A.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, Sch Phys & Astron, SUPA, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.; Volpi, G.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Aad, G.; Amoroso, S.; Barber, T.; Bernhard, R.; Boehler, M.; Bruneliere, R.; Christov, A.; Consorti, V.; Di Simone, A.; Fehling-Kaschek, M.; Flechl, M.; Giuliani, C.; Hartert, J.; Herten, G.; Jakobs, K.; Koneke, K.; Kononov, A. I.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Lohwasser, K.; Ludwig, I.; Ludwig, J.; Madar, R.; Mahboubi, K.; Mohr, W.; Parzefall, U.; Rammensee, M.; Rave, T. C.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Siegert, F.; Stoerig, K.; Sundermann, J. E.; Temming, K. K.; Thoma, S.; Tsiskaridze, V.; Ungaro, F. C.; Venturi, M.; Vivarelli, I.; von Radziewski, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Winkelmann, S.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Alexandre, G.; Backes, M.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Bucci, F.; Toro, R. Camacho; Clark, A.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Latour, B. Martin dit; Mermod, P.; Herrera, C. Mora; Muenstermann, D.; Nektarijevic, S.; Nikolics, K.; Pasztor, G.; Picazio, A.; Pohl, M.; Rosbach, K.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Beccherle, R.; Caso, C.; Darbo, G.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Barberis, D.; Caso, C.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Khubua, J.; Mchedlidze, G.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Duren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Bussey, P.; Buttar, C. M.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Edwards, N. C.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Quilty, D.; Ravenscroft, T.; Robson, A.; Saxon, D. H.; Smith, K. M.; Denis, R. D. St.; Steele, G.; Thompson, A. S.; Wraight, K.; Wright, M.] Univ Glasgow, Sch Phys & Astron, SUPA, Glasgow, Lanark, Scotland. [Bierwagen, K.; Blumenschein, U.; Brandt, O.; Evangelakou, D.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Hensel, C.; Kawamura, G.; Keil, M.; Knue, A.; Kohn, F.; Krieger, N.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Meyer, J.; Morel, J.; Nackenhorst, O.; Pashapour, S.; Peters, R. F. Y.; Quadt, A.; Roe, A.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Schroeder, T. Vazquez; Weingarten, J.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Brown, J.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] Univ Grenoble 1, Lab Phys Subatom & Cosmol, Grenoble, France. [Albrand, S.; Brown, J.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] CNRS, IN2P3, Grenoble, France. [Albrand, S.; Brown, J.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Le, B. T.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocme, B.] Inst Natl Polytech Grenoble, F-38031 Grenoble, France. [Addy, T. N.; Harvey, A.; McFarlane, K. W.; Shin, T.; Vassilakopoulos, V. I.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Belloni, A.; Butler, B.; Catastini, P.; Conti, G.; Franklin, M.; Huth, J.; Jeanty, L.; Kagan, M.; Mateos, D. Lopez; Mercurio, K. M.; Mills, C.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Yen, A. L.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Anders, G.; Andrei, V.; Davygora, Y.; Dietzsch, T. A.; Dunford, M.; Hanke, P.; Hofmann, J. I.; Khomich, A.; Kluge, E. -E.; Laier, H.; Lang, V. S.; Lendermann, V.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Kugel, A.; Schroer, N.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Evans, H.; Gagnon, P.; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Price, D.; Whittington, D.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Franz, S.; Jussel, P.; Kneringer, E.; Lukas, W.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Cinca, D.; Gandrajula, R. P.; Halladjian, G.; Limper, M.; Mallik, U.; Mandrysch, R.; Morange, N.; Pylypchenko, Y.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Ruiz-Martinez, A.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Aleksandrov, I. N.; Bardin, D. Y.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Grigalashvili, N.; Huseynov, N.; Karpov, S. N.; Kazarinov, M. Y.; Kharchenko, D.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rumyantsev, L.; Rusakovich, N. A.; Sadykov, R.; Shiyakova, M.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.; Zimin, N. I.] Joint Inst Nucl Res Dubna, Dubna, Russia. [Amako, K.; Arai, Y.; Doi, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Makida, Y.; Mitsui, S.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [King, M.; Kishimoto, T.; Kitamura, T.; Kurashige, H.; Matsushita, T.; Ochi, A.; Shimizu, S.; Takeda, H.; Tani, K.; Watanabe, I.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Sasao, N.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Verzini, M. J. Alconada; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Verzini, M. J. Alconada; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Allison, L. J.; Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Bianco, M.; Cataldi, G.; Gorini, E.; Grancagnolo, F.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Bianco, M.; Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Greenshaw, T.; Gwilliam, C. B.; Hayward, H. S.; Jackson, J. N.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Schnellbach, Y. J.; Sellers, G.; Vossebeld, J. H.; Waller, P.; Wrona, B.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia. [Bona, M.; Carter, A. A.; Cerrito, L.; Eisenhandler, E.; Ellis, K.; Fletcher, G.; Goddard, J. R.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Rizvi, E.; Salamanna, G.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Alam, M. A.; Berry, T.; Boisvert, V.; Brooks, T.; Cantrill, R.; Cooper-Smith, N. J.; Cowan, G.; Duguid, L.; Edwards, C. A.; George, S.; Gibson, S. M.; Goncalo, R.; Vazquez, J. G. Panduro; Pastore, Fr.; Rose, M.; Spano, F.; Strong, J. A.; Teixeira-Dias, P.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Baker, S.; Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christidi, I. A.; Cooper, B. D.; Davison, A. R.; Dobson, E.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Lambourne, L.; Nash, M.; Nurse, E.; Ochoa, M. I.; Pilkington, A. D.; Prabhu, R.; Sherwood, P.; Simmons, B.; Taylor, C.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Bernius, C.; Dhullipudi, R.; Greenwood, Z. D.; Sawyer, L.; Sircar, A.; Subramaniam, R.; Tamsett, M. C.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Jarlskog, G.; Lytken, E.; Meirose, B.; Mjoernmark, J. U.; Smirnova, O.; Wielers, M.] Lund Univ, Inst Fys, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De La Torre, H.; Del Peso, J.; Glasman, C.; Labarga, L.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Arnaez, O.; Blum, W.; Buscher, V.; Caputo, R.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Goeringer, C.; Handel, C.; Heck, T.; Hohlfeld, M.; Hsu, P. J.; Hulsing, T. A.; Ji, W.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Kopke, L.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Meyer, C.; Moreno, D.; Moritz, S.; Mueller, T.; Neusiedl, A.; Poettgen, R.; Sander, H. G.; Schafer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Almond, J.; Borri, M.; Brown, G.; Chavda, V.; Cox, B. E.; Da Via, C.; Forti, A.; Howarth, J.; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Marx, M.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Robinson, J. E. M.; Tomlinson, L.; Watts, S.; Woudstra, M. J.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Alio, L.; Barbero, M.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Nagai, Y.; Odier, J.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Alio, L.; Barbero, M.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Nagai, Y.; Odier, J.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Brau, B.; Colon, G.; Dallapiccola, C.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Dufour, M-A.; Klemetti, M.; Mantifel, R.; Robertson, S. H.; Schram, M.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Diglio, S.; Hamano, K.; Jennens, D.; Kubota, T.; Limosani, A.; Hanninger, G. Nunes; Phan, A.; Shao, Q. T.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Volpi, M.; White, M. J.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Armbruster, A. J.; Chapman, J. W.; Chelstowska, M. A.; Cirilli, M.; Dai, T.; Diehl, E. B.; Dubbert, J.; Feng, H.; Ferretti, C.; Goldfarb, S.; Harper, D.; Levin, D.; Li, X.; Liu, L.; Mc Kee, S. P.; Neal, H. A.; Panikashvili, N.; Qian, J.; Scheirich, D.; Searcy, J.; Thun, R. P.; Walch, S.; Wilson, A.; Wooden, G.; Wu, Y.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Hauser, R.; Hayden, D.; Holzbauer, J. L.; Huston, J.; Koll, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schwienhorst, R.; Stelzer, H. J.; Tollefson, K.; True, P.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alessandria, F.; Alimonti, G.; Andreazza, A.; Besana, M. I.; Broggi, F.; Carminati, L.; Cavalli, D.; Citterio, M.; Coelli, S.; Consonni, S. M.; Costa, G.; Fanti, M.; Favareto, A.; Giugni, D.; Koletsou, I.; Lari, T.; Mandelli, L.; Mazzanti, M.; Meloni, F.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Rivoltella, G.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Volpini, G.] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Andreazza, A.; Besana, M. I.; Carminati, L.; Consonni, S. M.; Fanti, M.; Favareto, A.; Meloni, F.; Perini, L.; Pizio, C.; Ragusa, F.; Rivoltella, G.; Simoniello, R.; Turra, R.] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Satsounkevitch, I.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus. [Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Asbah, N.; Azuelos, G.; Bouchami, J.; Dallaire, F.; Davies, M.; Gauthier, L.; Giunta, M.; Leroy, C.; Martin, J. P.; Rezvani, R.; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.] Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] ITEP, Moscow, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Romaniouk, A.; Shulga, E.; Smirnov, S. 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G.; Canale, V.; Carlino, G.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; della Volpe, D.; Di Donato, C.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Patricelli, S.; Sanchez, A.; Sekhniaidze, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Chiefari, G.; della Volpe, D.; Di Donato, C.; Giordano, R.; Merola, L.; Patricelli, S.; Sanchez, A.] Univ Naples Federico II, Dipartimento Sci Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Dao, V.; De Groot, N.; Filthaut, F.; Klok, P. F.; Konig, A. C.; Raas, M.; Salvucci, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Castelli, A.; Colijn, A. 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[Augsten, K.; Gallus, P.; Gunther, J.; Jakubek, J.; Kohout, Z.; Kral, V.; Pospisil, S.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solar, M.; Solc, J.; Sopko, V.; Sopko, B.; Stekl, I.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Torregrosa, E. Fullana; Kodys, P.; Leitner, R.; Novakova, J.; Pleskot, V.; Rybar, M.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.; Wilhelm, I.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Ammosov, V. V.; Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Ivashin, A. V.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] Inst High Energy Phys, State Res Ctr, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Gillman, A. R.; Haywood, S. J.; Kirk, J.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Tyndel, M.; Wickens, F. J.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Benslama, K.] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Shiga, Japan. [Anulli, F.; Artoni, G.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Pedis, D.; De Salvo, A.; De Zorzi, G.; Dionisi, C.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Rescigno, M.; Rosati, S.; Rossi, E.; Tehrani, F. Safai; Sidoti, A.; Camillocci, E. Solfaroli; Vari, R.; Veneziano, S.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma 1, Rome, Italy. [Artoni, G.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Zorzi, G.; Dionisi, C.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Rossi, E.; Camillocci, E. Solfaroli; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Liberti, B.; Marchese, F.; Mazzaferro, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Milan, Italy. [Aielli, G.; Camarri, P.; Cattani, G.; Di Ciaccio, A.; Marchese, F.; Mazzaferro, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Branchini, P.; Ceradini, F.; Di Luise, S.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Stanescu, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Luise, S.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Trovatelli, M.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.; Lablak, S.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA, Fac Sci Semlalia, Marrakech, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui] Univ Mohamed V Agdal, Fac Sci, Rabat, Morocco. [Abreu, H.; Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Bolnet, N. M.; Boonekamp, M.; Chevalier, L.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Grabas, H. M. X.; Guyot, C.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Legendre, M.; Maiani, C.; Mal, P.; Ramos, J. A. Manjarres; Mansoulie, B.; Martinez, H.; Meric, N.; Meyer, J-P.; Mijovic, L.; Hong, V. Nguyen Thi; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Resende, B.; Royon, C. R.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.; Tsionou, D.; Vranjes, N.; Xiao, M.] CEA Saclay, DSM IRFU, F-91191 Gif Sur Yvette, France. [Damiani, D. S.; Grillo, A. A.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Mitrevski, J.; Nielsen, J.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Beckingham, M.; Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Hsu, S. -C.; Keller, J. S.; Lubatti, H. J.; Rompotis, N.; Rothberg, J.; Verducci, M.; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Paredes, B. Lopez; Mcfayden, J. A.; Miyagawa, P. S.; Owen, S.; Paganis, E.; Suruliz, K.; Tovey, D. R.; Tua, A.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Ibragimov, I.; Ikematsu, K.; Rammes, M.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Dawe, E.; Godfrey, J.; Kvita, J.; O'Neil, D. C.; Petteni, M.; Stelzer, B.; Tanasijczuk, A. J.; Trottier-McDonald, M.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Mayes, J. Backus; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Hansson, P.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nelson, T. 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[Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. 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[Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Coggeshall, J.; Cortes-Gonzalez, A.; Errede, D.; Errede, S.; Lie, K.; Liss, T. M.; McCarn, A.; Neubauer, M. S.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Brenner, R.; Buszello, C. P.; Coniavitis, E.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Pelikan, D.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Moya, M. Minao; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. 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Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Moya, M. Minao; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Moya, M. Minao; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. 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RI KHODINOV, ALEKSANDR/D-6269-2015; Goncalo, Ricardo/M-3153-2016; Gauzzi, Paolo/D-2615-2009; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Yang, Haijun/O-1055-2015; Monzani, Simone/D-6328-2017; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Olshevskiy, Alexander/I-1580-2016; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Mora Herrera, Maria Clemencia/L-3893-2016; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; Doyle, Anthony/C-5889-2009; Marti-Garcia, Salvador/F-3085-2011; Brooks, William/C-8636-2013; Boyko, Igor/J-3659-2013; Moraes, Arthur/F-6478-2010; Ferrando, James/A-9192-2012; Solfaroli Camillocci, Elena/J-1596-2012; Snesarev, Andrey/H-5090-2013; Warburton, Andreas/N-8028-2013; Turchikhin, Semen/O-1929-2013; Sukharev, Andrey/A-6470-2014; Akimov, Andrey/N-1769-2015; Tikhomirov, Vladimir/M-6194-2015; Chekulaev, Sergey/O-1145-2015; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; Andreazza, Attilio/E-5642-2011; Carvalho, Joao/M-4060-2013; Mashinistov, Ruslan/M-8356-2015; Buttar, Craig/D-3706-2011; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Della Pietra, Massimo/J-5008-2012; Cavalli-Sforza, Matteo/H-7102-2015; Petrucci, Fabrizio/G-8348-2012; Negrini, Matteo/C-8906-2014; Ferrer, Antonio/H-2942-2015; Hansen, John/B-9058-2015; Grancagnolo, Sergio/J-3957-2015; spagnolo, stefania/A-6359-2012; Ciubancan, Liviu Mihai/L-2412-2015; Shmeleva, Alevtina/M-6199-2015; Camarri, Paolo/M-7979-2015; Gavrilenko, Igor/M-8260-2015; Grinstein, Sebastian/N-3988-2014; Wemans, Andre/A-6738-2012; Demirkoz, Bilge/C-8179-2014; Gutierrez, Phillip/C-1161-2011; Ventura, Andrea/A-9544-2015; Livan, Michele/D-7531-2012; De, Kaushik/N-1953-2013; Mitsou, Vasiliki/D-1967-2009; White, Ryan/E-2979-2015; Joergensen, Morten/E-6847-2015; Riu, Imma/L-7385-2014; Mir, Lluisa-Maria/G-7212-2015; Staroba, Pavel/G-8850-2014; Kupco, Alexander/G-9713-2014; de Groot, Nicolo/A-2675-2009; Hejbal, Jiri/H-1358-2014; Marcisovsky, Michal/H-1533-2014; Mikestikova, Marcela/H-1996-2014; Lysak, Roman/H-2995-2014; Tomasek, Lukas/G-6370-2014; Svatos, Michal/G-8437-2014; Chudoba, Jiri/G-7737-2014; Peleganchuk, Sergey/J-6722-2014; Bosman, Martine/J-9917-2014; Castro, Nuno/D-5260-2011; Lee, Jason/B-9701-2014; Robson, Aidan/G-1087-2011; Kuday, Sinan/C-8528-2014; Smirnova, Oxana/A-4401-2013; Gabrielli, Alessandro/H-4931-2012; Zimmermann, Claus/E-9598-2014; Fabbri, Laura/H-3442-2012; Villa, Mauro/C-9883-2009; Nozka, Libor/G-5550-2014; Nemecek, Stanislav/G-5931-2014; Kepka, Oldrich/G-6375-2014; Lokajicek, Milos/G-7800-2014; Jakoubek, Tomas/G-8644-2014 OI KHODINOV, ALEKSANDR/0000-0003-3551-5808; Goncalo, Ricardo/0000-0002-3826-3442; Gauzzi, Paolo/0000-0003-4841-5822; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Monzani, Simone/0000-0002-0479-2207; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Vykydal, Zdenek/0000-0003-2329-0672; Olshevskiy, Alexander/0000-0002-8902-1793; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; Doyle, Anthony/0000-0001-6322-6195; Brooks, William/0000-0001-6161-3570; Boyko, Igor/0000-0002-3355-4662; Moraes, Arthur/0000-0002-5157-5686; Ferrando, James/0000-0002-1007-7816; Solfaroli Camillocci, Elena/0000-0002-5347-7764; Warburton, Andreas/0000-0002-2298-7315; Turchikhin, Semen/0000-0001-6506-3123; Tikhomirov, Vladimir/0000-0002-9634-0581; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; Andreazza, Attilio/0000-0001-5161-5759; Carvalho, Joao/0000-0002-3015-7821; Mashinistov, Ruslan/0000-0001-7925-4676; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Della Pietra, Massimo/0000-0003-4446-3368; Petrucci, Fabrizio/0000-0002-5278-2206; Negrini, Matteo/0000-0003-0101-6963; Ferrer, Antonio/0000-0003-0532-711X; Hansen, John/0000-0002-8422-5543; Grancagnolo, Sergio/0000-0001-8490-8304; spagnolo, stefania/0000-0001-7482-6348; Ciubancan, Liviu Mihai/0000-0003-1837-2841; Camarri, Paolo/0000-0002-5732-5645; Grinstein, Sebastian/0000-0002-6460-8694; Wemans, Andre/0000-0002-9669-9500; Ventura, Andrea/0000-0002-3368-3413; Livan, Michele/0000-0002-5877-0062; De, Kaushik/0000-0002-5647-4489; Mitsou, Vasiliki/0000-0002-1533-8886; White, Ryan/0000-0003-3589-5900; Joergensen, Morten/0000-0002-6790-9361; Riu, Imma/0000-0002-3742-4582; Mir, Lluisa-Maria/0000-0002-4276-715X; Mikestikova, Marcela/0000-0003-1277-2596; Tomasek, Lukas/0000-0002-5224-1936; Svatos, Michal/0000-0002-7199-3383; Peleganchuk, Sergey/0000-0003-0907-7592; Bosman, Martine/0000-0002-7290-643X; Castro, Nuno/0000-0001-8491-4376; Lee, Jason/0000-0002-2153-1519; Kuday, Sinan/0000-0002-0116-5494; Smirnova, Oxana/0000-0003-2517-531X; Gabrielli, Alessandro/0000-0001-5346-7841; Fabbri, Laura/0000-0002-4002-8353; Villa, Mauro/0000-0002-9181-8048; FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union; ERC, European Union; NSRF, European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; ISF, Israel; MINERVA, Israel; GIF, Israel; DIP, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; GRICES, Portugal; FCT, Portugal; MERYS (MECTS), Romania; MES of Russia, Russian Federation; ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MVZT, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC, and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST, and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR, and VSC CR, Czech Republic; DNRF, DNSRC, and Lundbeck Foundation, Denmark; EPLANET, ERC, and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG, and AvH Foundation, Germany; GSRT and NSRF, Greece; ISF, MINERVA, GIF, DIP, and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW, Poland; GRICES and FCT, Portugal; MERYS (MECTS), Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MVZT, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF, and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular, from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CCIN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK), and BNL (USA) and in the Tier-2 facilities worldwide. NR 30 TC 23 Z9 23 U1 8 U2 157 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 9 PY 2013 VL 111 IS 15 AR 152301 DI 10.1103/PhysRevLett.111.152301 PG 18 WC Physics, Multidisciplinary SC Physics GA 239UA UT WOS:000326050000002 PM 24160592 ER PT J AU Jin, LX Mathur, R Rother, G Cole, D Bazilevskaya, E Williams, J Carone, A Brantley, S AF Jin, Lixin Mathur, Ryan Rother, Gernot Cole, David Bazilevskaya, Ekaterina Williams, Jennifer Carone, Alex Brantley, Susan TI Evolution of porosity and geochemistry in Marcellus Formation black shale during weathering SO CHEMICAL GEOLOGY LA English DT Article DE Pyrite dissolution; Organic matter; Shale gas; Trace metals; Neutron scattering; Computed tomography ID ANGLE NEUTRON-SCATTERING; ORGANIC-CARBON; APPALACHIAN BASIN; COMPUTED-TOMOGRAPHY; SURFACE-AREA; ALBANY SHALE; ROCKS; ELEMENTS; REGOLITH; MOBILITY AB Soils developed on the Oatka Creek member of the Marcellus Formation in Huntingdon, Pennsylvania were analyzed to understand the evolution of black shale matrix porosity and the associated changes in elemental and mineralogical composition during infiltration of water into organic-rich shale. Making the reasonable assumption that soil erosion rates are the same as those measured in a nearby location on a less organic-rich shale, we suggest that soil production rates have on average been faster for this black shale compared to the gray shale in similar climate settings. This difference is attributed to differences in composition: both shales are dominantly quartz, illite, and chlorite, but the Oatka Creek member at this location has more organic matter (1.25 wt.% organic carbon in rock fragments recovered from the bottom of the auger cores and nearby outcrops) and accessory pyrite. During weathering, the extremely low-porosity bedrock slowly disaggregates into shale chips with intergranular pores and fractures. Some of these pores are either filled with organic matter or air-filled but remain unconnected, and thus inaccessible to water. Based on weathering bedrock/soil profiles, disintegration is initiated with oxidation of pyrite and organic matter, which increases the overall porosity and most importantly allows water penetration. Water infiltration exposes fresh surface area and thus promotes dissolution of plagioclase and clays. As these dissolution reactions proceed, the porosity in the deepest shale chips recovered from the soil decrease from 9 to 7% while kaolinite and Fe oxyhydroxides precipitate. Eventually, near the land surface, mineral precipitation is outcompeted by dissolution or particle loss of illite and chlorite and porosity in shale chips increases to 20%. As imaged by computed tomographic analysis, weathering causes i) greater porosity, ii) greater average length of connected pores, and iii) a more branched pore network compared to the unweathered sample. This work highlights the impact of shale-water-O-2 interactions in near-surface environments: (1) black shale weathering is important for global carbon cycles as previously buried organic matter is quickly oxidized; and (2) black shales weather more quickly than less organic-and sulfide-rich shales, leading to high porosity and mineral surface areas exposed for clay weathering. The fast rates of shale gas exploitation that are ongoing in Pennsylvania, Texas and other regions in the United States may furthermore lead to release of metals to the environment if reactions between water and black shale are accelerated by gas development activities in the subsurface just as they are by low-temperature processes in our field study. (C) 2013 Elsevier B.V. All rights reserved. C1 [Jin, Lixin] Univ Texas El Paso, Dept Geol Sci, El Paso, TX 79968 USA. [Jin, Lixin; Bazilevskaya, Ekaterina; Williams, Jennifer; Brantley, Susan] Penn State Univ, Earth & Environm Syst Inst, University Pk, PA 16803 USA. [Carone, Alex; Brantley, Susan] Penn State Univ, Dept Geosci, University Pk, PA 16803 USA. [Mathur, Ryan] Juniata Coll, Dept Geol, Huntingdon, PA 16652 USA. [Rother, Gernot] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Cole, David] Ohio State Univ, Dept Geol Sci, Columbus, OH 43210 USA. RP Jin, LX (reprint author), Univ Texas El Paso, Dept Geol Sci, El Paso, TX 79968 USA. EM ljin2@utep.edu RI Rother, Gernot/B-7281-2008 OI Rother, Gernot/0000-0003-4921-6294 FU Susquehanna-Shale Hills Critical Zone Observatory [NSF-EAR-0725019]; Department of Energy Grant [DE-FG02-05ER15675]; National Science Foundation [DMR-0944772]; Department of Energy Office of Science Basic Energy Sciences Energy Frontier Research Center - Nanoscale Control of Geologic; Division of Chemical Sciences, Geosciences and Biosciences, Office of Basic Energy Science, US Department of Energy FX We acknowledge A. Dere, A. Fornadel, J. Paul, V. Prush, C. Ebersole, J. Kaye and K. Downie for soil sample collection and analyses, and H. Gong, L. Liermann and W. Castro for ICP AES and ICP MS analyses. We acknowledge support from the Susquehanna-Shale Hills Critical Zone Observatory (NSF-EAR-0725019 to C. Duffy, Penn State) and from the Department of Energy Grant (DE-FG02-05ER15675 to SLB), and neutron scattering instrumentation and technical support from David Mildner at NIST-NCNR. The research using the small-angle scattering instruments at the National Institute of Standards and Technology was supported in part by the National Science Foundation under Agreement No. DMR-0944772. DRC was supported by the Department of Energy Office of Science Basic Energy Sciences Energy Frontier Research Center - Nanoscale Control of Geologic CO2. GR's effort was sponsored by the Division of Chemical Sciences, Geosciences and Biosciences, Office of Basic Energy Science, US Department of Energy. NR 80 TC 21 Z9 24 U1 7 U2 122 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2541 EI 1878-5999 J9 CHEM GEOL JI Chem. Geol. PD OCT 9 PY 2013 VL 356 BP 50 EP 63 DI 10.1016/j.chemgeo.2013.07.012 PG 14 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA 242HP UT WOS:000326230100005 ER PT J AU Tsang, T Gassner, D Minty, M AF Tsang, T. Gassner, D. Minty, M. TI Residual gas fluorescence monitor for relativistic heavy ions at RHIC SO PHYSICAL REVIEW SPECIAL TOPICS-ACCELERATORS AND BEAMS LA English DT Article AB A residual gas fluorescence beam profile monitor at the Relativistic Heavy Ion Collider (RHIC) has successfully recorded beam images of various species of relativistic heavy ions during FY2012 operations. These fully striped ions include gold, copper, and uranium at 100, 99.9, and 96: 4 GeV/n, respectively. Their beam profiles give an independent measurement of the RHIC beam size and emittance. We estimated their corresponding fluorescence cross sections to be 2.1 x 10(-16), 1.8 x 10(-17), and 2.6 x 10(-16) cm(2), and obtained their rms transverse beam sizes of 0.36, 0.37, 0.24 mm for gold, copper, and uranium ions, respectively. They are the smallest ion beam width, thus lowest beam emittance, ever produced at RHIC or any other high-energy heavy ion colliders. These extremely small beam sizes may have reached a fundamental limit to residual gas fluorescence based beam profile monitor. Nevertheless, this beam diagnostic technique, utilizing the beam-induced fluorescence from residual gas where hydrogen is still the dominant constituent in nearly all vacuum systems, represents a passive, robust, truly noninvasive, monitor for high-energy ion beams. C1 [Tsang, T.] Brookhaven Natl Lab, Instrumentat Div, Upton, NY 11973 USA. [Gassner, D.; Minty, M.] Brookhaven Natl Lab, Collider Accelerator Div, Upton, NY 11973 USA. RP Tsang, T (reprint author), Brookhaven Natl Lab, Instrumentat Div, Upton, NY 11973 USA. EM Tsang@bnl.gov FU U.S. Department of Energy [DE-AC02-98CH10886] FX This work was supported by U.S. Department of Energy under Contract No. DE-AC02-98CH10886. NR 12 TC 1 Z9 1 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-4402 J9 PHYS REV SPEC TOP-AC JI Phys. Rev. Spec. Top.-Accel. Beams PD OCT 9 PY 2013 VL 16 IS 10 AR 102802 DI 10.1103/PhysRevSTAB.16.102802 PG 7 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA 241EI UT WOS:000326148800003 ER PT J AU del Campo, A Kibble, TWB Zurek, WH AF del Campo, A. Kibble, T. W. B. Zurek, W. H. TI Causality and non-equilibrium second-order phase transitions in inhomogeneous systems SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article ID COSMOLOGICAL EXPERIMENTS; SUPERFLUID HE-3; DYNAMICS; SIMULATION; UNIVERSE; STRINGS AB When a second-order phase transition is crossed at a finite rate, the evolution of the system stops being adiabatic as a result of the critical slowing down in the neighborhood of the critical point. In systems with a topologically nontrivial vacuum manifold, disparate local choices of the ground state lead to the formation of topological defects. The universality class of the transition imprints a signature on the resulting density of topological defects: it obeys a power law in the quench rate, with an exponent dictated by a combination of the critical exponents of the transition. In inhomogeneous systems the situation is more complicated, as the spontaneous symmetry breaking competes with bias caused by the influence of the nearby regions that already chose the new vacuum. As a result, the choice of the broken symmetry vacuum may be inherited from the neighboring regions that have already entered the new phase. This competition between the inherited and spontaneous symmetry breaking enhances the role of causality, as the defect formation is restricted to a fraction of the system where the front velocity surpasses the relevant sound velocity and phase transition remains effectively homogeneous. As a consequence, the overall number of topological defects can be substantially suppressed. When the fraction of the system is small, the resulting total number of defects is still given by a power law related to the universality class of the transition, but exhibits a more pronounced dependence on the quench rate. This enhanced dependence complicates the analysis but may also facilitate experimental testing of defect formation theories. C1 [del Campo, A.; Zurek, W. H.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [del Campo, A.] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. [Kibble, T. W. B.] Univ London Imperial Coll Sci Technol & Med, Blackett Lab, London SW7 2AZ, England. RP del Campo, A (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM delcampo@lanl.gov RI del Campo, Adolfo/B-8439-2009; OI del Campo, Adolfo/0000-0003-2219-2851; Kibble, Thomas/0000-0001-7667-0260 FU US Department of Energy through LANL/LDRD Program; US Department of Energy through LANL J Robert Oppenheimer fellowship FX It is a pleasure to thank Tanja E Mehlstaubler for facilitating the snapshots of ion chains used in figure 4, Brian P Anderson for the pictures of growing Bose-Einstein condensates supporting vortices reported in figure 6, and Marek M Rams for the numerical data in figure 3(b). We further thank Bogdan Damski and Marek M Rams for useful suggestions, and Emilie Passemar for help in editing the figures. This research is supported by the US Department of Energy through the LANL/LDRD Program and a LANL J Robert Oppenheimer fellowship (AdC). NR 65 TC 20 Z9 20 U1 0 U2 10 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD OCT 9 PY 2013 VL 25 IS 40 AR 404210 DI 10.1088/0953-8984/25/40/404210 PG 10 WC Physics, Condensed Matter SC Physics GA 221HI UT WOS:000324648200011 PM 24025443 ER PT J AU Ekuma, CE Lin, CH Moreno, J Ku, W Jarrell, M AF Ekuma, Chinedu E. Lin, Chia-Hui Moreno, Juana Ku, Wei Jarrell, Mark TI First-principlesWannier function analysis of the electronic structure of PdTe: weaker magnetism and superconductivity SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article ID TELLURIDES; PALLADIUM AB We report a first-principles Wannier function study of the electronic structure of PdTe. Its electronic structure is found to be a broad three-dimensional Fermi surface with highly reduced correlation effects. In addition, the higher filling of the Pd d-shell, its stronger covalency resulting from the closer energy of the Pd d and Te p shells, and the larger crystal field effects of the Pd ion due to its near octahedral coordination, all serve to weaken significantly electronic correlations in the particle-hole (spin, charge, and orbital) channel. In comparison to the Fe chalcogenides, e. g. FeSe, we highlight the essential features (quasi-two-dimensionality, proximity to half-filling, weaker covalency, and higher orbital degeneracy) of Fe-based high-temperature superconductors. C1 [Ekuma, Chinedu E.; Moreno, Juana; Jarrell, Mark] Louisiana State Univ, Dept Phys & Astron, Baton Rouge, LA 70803 USA. [Ekuma, Chinedu E.; Moreno, Juana; Jarrell, Mark] Louisiana State Univ, Ctr Computat & Technol, Baton Rouge, LA 70803 USA. [Lin, Chia-Hui; Ku, Wei] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Lin, Chia-Hui; Ku, Wei] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RP Ekuma, CE (reprint author), Louisiana State Univ, Dept Phys & Astron, Baton Rouge, LA 70803 USA. EM cekuma1@lsu.edu RI Moreno, Juana/D-5882-2012 FU National Science Foundation LA-SiGMA award [EPS 1003897]; US Department of Energy (DOE) [DE-AC02-98CH10886]; DOE-CMCSN [DE-AC02-98CH10886] FX We thank Carol Duran for carefully reading the manuscript. Work at LSU is funded by the National Science Foundation LA-SiGMA award: EPS 1003897. Work at BNL is supported by the US Department of Energy (DOE) under contract DE-AC02-98CH10886. Inter-institutional collaboration is supported by the DOE-CMCSN grant DE-AC02-98CH10886. High performance computational resources are provided by the Louisiana Optical Network Initiative (LONI) and Brookhaven National Laboratory (BNL) clusters. NR 57 TC 4 Z9 4 U1 1 U2 17 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD OCT 9 PY 2013 VL 25 IS 40 AR 405601 DI 10.1088/0953-8984/25/40/405601 PG 6 WC Physics, Condensed Matter SC Physics GA 221HI UT WOS:000324648200020 PM 24025790 ER PT J AU Zurek, WH AF Zurek, W. H. TI Topological relics of symmetry breaking: winding numbers and scaling tilts from random vortex-antivortex pairs SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article ID DEFECT FORMATION; COSMOLOGICAL EXPERIMENTS; PHASE-TRANSITIONS; COSMIC STRINGS; SUPERFLUID; CRYSTALS; DYNAMICS AB I show that random distributions of vortex-antivortex pairs (rather than of individual vortices) lead to scaling of typical winding numbers W trapped inside a loop of circumference C with the square root of that circumference, W similar to root C, when the expected winding numbers are large, vertical bar W vertical bar >> 1. Such scaling is consistent with the Kibble-Zurek mechanism (KZM), with < W-2 > inversely proportional to (xi) over cap, the typical size of the domain that can break symmetry in unison. (The dependence of (xi) over cap on quench rate is predicted by KZM from critical exponents of the phase transition.) Thus, according to KZM, the dispersion root < W-2 > scales as root C/(xi) over cap for large W. By contrast, a distribution of individual vortices with randomly assigned topological charges would result in the dispersion scaling with the square root of the area inside C (i.e., root < W-2 > similar to C). Scaling of the dispersion of W as well as of the probability of detection of non-zero W with C and (xi) over cap can be also studied for loops so small that non-zero windings are rare. In this case I show that dispersion varies not as 1/root(xi) over cap, but as 1/(xi) over cap, which results in a doubling of the scaling of dispersion with the quench rate when compared to the large vertical bar W vertical bar regime. Moreover, the probability of trapping of non-zero W becomes approximately equal to < W-2 >, and scales as 1/(xi) over cap (2). This quadruples-as compared with root < W-2 > similar or equal to root C/(xi) over cap valid for large W-the exponent in the power law dependence of the frequency of trapping of vertical bar W vertical bar = 1 on (xi) over cap when the probability of vertical bar W vertical bar > 1 is negligible. This change of the power law exponent by a factor of four-from 1/root(xi) over cap for the dispersion of large W to 1/(xi) over cap (2) for the frequency of non-zero W when vertical bar W vertical bar > 1 is negligibly rare-is of paramount importance for experimental tests of KZM. C1 Los Alamos Natl Lab, Div Theory, Los Alamos, NM 87545 USA. RP Zurek, WH (reprint author), Los Alamos Natl Lab, Div Theory, Los Alamos, NM 87545 USA. FU Department of Energy FX Discussions with Sang-Wook Cheong, Adolfo del Campo, Jacek Dziarmaga, Valery Kiryukhin, Raymond Rivers and Vivien Zapf are gratefully acknowledged. This work was supported by the Department of Energy through the LDRD program in Los Alamos. NR 39 TC 2 Z9 2 U1 0 U2 6 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD OCT 9 PY 2013 VL 25 IS 40 AR 404209 DI 10.1088/0953-8984/25/40/404209 PG 8 WC Physics, Condensed Matter SC Physics GA 221HI UT WOS:000324648200010 PM 24025395 ER PT J AU Ji, CR Melnitchouk, W Thomas, AW AF Ji, Chueng-Ryong Melnitchouk, W. Thomas, A. W. TI Anatomy of relativistic pion loop corrections to the electromagnetic nucleon coupling SO PHYSICAL REVIEW D LA English DT Article ID CHIRAL PERTURBATION-THEORY; SCATTERING LENGTHS; SYMMETRY-BREAKING; FLAVOR ASYMMETRY; MATRIX-ELEMENTS; VECTOR CURRENT; FORM-FACTORS; SEA; PROTON; DYNAMICS AB We present a relativistic formulation of pion loop corrections to the coupling of photons with nucleons on the light front. Vertex and wave function renormalization constants are computed to lowest order in the pion field, including their nonanalytic behavior in the chiral limit, and studied numerically as a function of the ultraviolet cutoff. Particular care is taken to explicitly verify gauge invariance and Ward-Takahashi identity constraints to all orders in the m(pi) expansion. The results are used to compute the chiral corrections to matrix elements of local operators, related to moments of deep-inelastic structure functions. Finally, comparison of results for pseudovector and pseudoscalar coupling allows the resolution of a longstanding puzzle in the computation of pion cloud corrections to structure function moments. C1 [Ji, Chueng-Ryong] N Carolina State Univ, Dept Phys, Raleigh, NC 27692 USA. [Melnitchouk, W.] Jefferson Lab, Newport News, VA 23606 USA. [Thomas, A. W.] Univ Adelaide, Sch Chem & Phys, CSSM, Adelaide, SA 5005, Australia. [Thomas, A. W.] Univ Adelaide, Sch Chem & Phys, CoEPP, Adelaide, SA 5005, Australia. RP Ji, CR (reprint author), N Carolina State Univ, Dept Phys, Raleigh, NC 27692 USA. RI Thomas, Anthony/G-4194-2012 OI Thomas, Anthony/0000-0003-0026-499X FU DOE [DE-AC05-06OR23177, DE-FG02-03ER41260]; Australian Research Council through the ARC Centre of Excellence for Particle Physics at the Terascale [FL0992247] FX We thank M. Birse, M. Burkardt, K. Hendricks, V. Lyubovitskij, M. Polyakov, and A.A. Vladimirov for helpful discussions. This work was supported by the DOE Contract No. DE-AC05-06OR23177, under which Jefferson Science Associates, LLC operates Jefferson Lab, DOE Contract No. DE-FG02-03ER41260, and the Australian Research Council through the ARC Centre of Excellence for Particle Physics at the Terascale and Grant FL0992247. NR 51 TC 10 Z9 10 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 EI 1550-2368 J9 PHYS REV D JI Phys. Rev. D PD OCT 9 PY 2013 VL 88 IS 7 AR 076005 DI 10.1103/PhysRevD.88.076005 PG 18 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 239PS UT WOS:000326038500003 ER PT J AU Adolph, C Alekseev, MG Alexakhin, VY Alexandrov, Y Alexeev, GD Amoroso, A Austregesilo, A Badelek, B Balestra, F Barth, J Baum, G Bedfer, Y Berlin, A Bernhard, J Bertini, R Bicker, K Bieling, J Birsa, R Bisplinghoff, J Bordalo, P Bradamante, F Braun, C Bravar, A Bressan, A Buchele, M Burtin, E Capozza, L Chiosso, M Chung, SU Cicuttin, A Crespo, ML Dalla Torre, S Dasgupta, SS Dasgupta, S Denisov, OY Donskov, SV Doshita, N Duic, V Dunnweber, W Dziewiecki, M Efremov, A Elia, C Eversheim, PD Eyrich, W Faessler, M Ferrero, A Filin, A Finger, M Finger, M Fischer, H Franco, C von Hohenesche, ND Friedrich, JM Frolov, V Garfagnini, R Gautheron, F Gavrichtchouk, OP Gerassimov, S Geyer, R Giorgi, M Gnesi, I Gobbo, B Goertz, S Grabmuller, S Grasso, A Grube, B Gushterski, R Guskov, A Guthorl, T Haas, F von Harrach, D Heinsius, FH Herrmann, F Hess, C Hinterberger, F Hoppner, C Horikawa, N d'Hose, N Huber, S Ishimoto, S Ivanshin, Y Iwata, T Jahn, R Jary, V Jasinski, P Joosten, R Kabuss, E Kang, D Ketzer, B Khaustov, GV Khokhlov, YA Kisselev, Y Klein, F Klimaszewski, K Koivuniemi, JH Kolosov, VN Kondo, K Konigsmann, K Konorov, I Konstantinov, VF Kotzinian, AM Kouznetsov, O Kramer, M Kroumchtein, ZV Kuchinski, N Kunne, F Kurek, K Kurjata, RP Lednev, AA Lehmann, A Levorato, S Lichtenstadt, J Maggiora, A Magnon, A Makke, N Mallot, GK Mann, A Marchand, C Martin, A Marzec, J Matsuda, H Matsuda, T Meshcheryakov, G Meyer, W Michigami, T Mikhailov, YV Miyachi, Y Morreale, A Nagaytsev, IA Nagel, T Nerling, F Neubert, S Neyret, D Nikolaenko, VI Novy, J Nowak, WD Nunes, AS Olshevsky, AG Ostrick, M Panknin, R Panzieri, D Parsamyan, B Paul, S Piragino, G Platchkov, S Pochodzalla, J Polak, J Polyakov, VA Pretz, J Quaresma, M Quintans, C Ramos, S Reicherz, G Rocco, E Rodionov, V Rondio, E Rossiyskaya, NS Ryabchikov, DI Samoylenko, VD Sandacz, A Sapozhnikov, MG Sarkar, S Savin, IA Sbrizzai, G Schiavon, P Schill, C Schluter, T Schmidt, A Schmidt, K Schmitt, L Schmiden, H Schonning, K Schopferer, S Schott, M Shevchenko, OY Silva, L Sinha, L Sirtl, S Sosio, S Sozzi, F Srnka, A Steiger, L Stolarski, M Sulc, M Sulej, R Suzuki, H Sznajder, P Takekawa, S Ter Wolbeek, J Tessaro, S Tessarotto, F Thibaud, F Uhl, S Uman, I Vandenbroucke, M Virius, M Wang, L Weisrock, T Wilfert, M Windmolders, R Wislicki, W Wollny, H Zaremba, K Zavertyaev, M Zemlyanichkina, E Zhuravlev, N Ziembicki, M AF Adolph, C. Alekseev, M. G. Alexakhin, V. Y. Alexandrov, Y. Alexeev, G. D. Amoroso, A. Austregesilo, A. Badelek, B. Balestra, F. Barth, J. Baum, G. Bedfer, Y. Berlin, A. Bernhard, J. Bertini, R. Bicker, K. Bieling, J. Birsa, R. Bisplinghoff, J. Bordalo, P. Bradamante, F. Braun, C. Bravar, A. Bressan, A. Buechele, M. Burtin, E. Capozza, L. Chiosso, M. Chung, S. U. Cicuttin, A. Crespo, M. L. Dalla Torre, S. Dasgupta, S. S. Dasgupta, S. Denisov, O. Y. Donskov, S. V. Doshita, N. Duic, V. Duennweber, W. Dziewiecki, M. Efremov, A. Elia, C. Eversheim, P. D. Eyrich, W. Faessler, M. Ferrero, A. Filin, A. Finger, M. Finger, M., Jr. Fischer, H. Franco, C. von Hohenesche, N. du Fresne Friedrich, J. M. Frolov, V. Garfagnini, R. Gautheron, F. Gavrichtchouk, O. P. Gerassimov, S. Geyer, R. Giorgi, M. Gnesi, I. Gobbo, B. Goertz, S. Grabmueller, S. Grasso, A. Grube, B. Gushterski, R. Guskov, A. Guthoerl, T. Haas, F. von Harrach, D. Heinsius, F. H. Herrmann, F. Hess, C. Hinterberger, F. Hoeppner, C. Horikawa, N. d'Hose, N. Huber, S. Ishimoto, S. Ivanshin, Y. Iwata, T. Jahn, R. Jary, V. Jasinski, P. Joosten, R. Kabuss, E. Kang, D. Ketzer, B. Khaustov, G. V. Khokhlov, Y. A. Kisselev, Y. Klein, F. Klimaszewski, K. Koivuniemi, J. H. Kolosov, V. N. Kondo, K. Koenigsmann, K. Konorov, I. Konstantinov, V. F. Kotzinian, A. M. Kouznetsov, O. Kraemer, M. Kroumchtein, Z. V. Kuchinski, N. Kunne, F. Kurek, K. Kurjata, R. P. Lednev, A. A. Lehmann, A. Levorato, S. Lichtenstadt, J. Maggiora, A. Magnon, A. Makke, N. Mallot, G. K. Mann, A. Marchand, C. Martin, A. Marzec, J. Matsuda, H. Matsuda, T. Meshcheryakov, G. Meyer, W. Michigami, T. Mikhailov, Y. V. Miyachi, Y. Morreale, A. Nagaytsev, I. A. Nagel, T. Nerling, F. Neubert, S. Neyret, D. Nikolaenko, V. I. Novy, J. Nowak, W. -D. Nunes, A. S. Olshevsky, A. G. Ostrick, M. Panknin, R. Panzieri, D. Parsamyan, B. Paul, S. Piragino, G. Platchkov, S. Pochodzalla, J. Polak, J. Polyakov, V. A. Pretz, J. Quaresma, M. Quintans, C. Ramos, S. Reicherz, G. Rocco, E. Rodionov, V. Rondio, E. Rossiyskaya, N. S. Ryabchikov, D. I. Samoylenko, V. D. Sandacz, A. Sapozhnikov, M. G. Sarkar, S. Savin, I. A. Sbrizzai, G. Schiavon, P. Schill, C. Schlueter, T. Schmidt, A. Schmidt, K. Schmitt, L. Schmiden, H. Schoenning, K. Schopferer, S. Schott, M. Shevchenko, O. Y. Silva, L. Sinha, L. Sirtl, S. Sosio, S. Sozzi, F. Srnka, A. Steiger, L. Stolarski, M. Sulc, M. Sulej, R. Suzuki, H. Sznajder, P. Takekawa, S. Ter Wolbeek, J. Tessaro, S. Tessarotto, F. Thibaud, F. Uhl, S. Uman, I. Vandenbroucke, M. Virius, M. Wang, L. Weisrock, T. Wilfert, M. Windmolders, R. Wislicki, W. Wollny, H. Zaremba, K. Zavertyaev, M. Zemlyanichkina, E. Zhuravlev, N. Ziembicki, M. TI Study of Sigma(1385) and Xi(1321) hyperon and antihyperon production in deep inelastic muon scattering SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID CHARGED CURRENT INTERACTIONS; NOMAD EXPERIMENT; (LAMBDA)OVER-BAR POLARIZATION; COMPASS; LAMBDA AB Large samples of Lambda, Sigma(1385) and Xi(1321) hyperons produced in the deep-inelastic muon scattering off a (LiD)-Li-6 target were collected with the COMPASS experimental setup at CERN. The relative yields of Sigma(1385)(+), Sigma(1385)(-), Sigma(1385)(-), Sigma(1385)(+), Xi(1321)(-), and Xi(1321)(+) hyperons decaying into Lambda(Lambda)pi were measured. The ratios of heavy-hyperon to Lambda and heavy-antihyperon to Lambda were found to be in the range 3.8 % to 5.6 % with a relative uncertainty of about 10 %. They were used to tune the parameters relevant for strange particle production of the LEPTO Monte Carlo generator. C1 [Baum, G.] Univ Bielefeld, Fak Phys, D-33501 Bielefeld, Germany. [Berlin, A.; Gautheron, F.; Hess, C.; Kisselev, Y.; Koivuniemi, J. H.; Meyer, W.; Reicherz, G.; Wang, L.] Ruhr Univ Bochum, Inst Expt Phys, D-44780 Bochum, Germany. [Bisplinghoff, J.; Eversheim, P. D.; Hinterberger, F.; Jahn, R.; Joosten, R.; Schmiden, H.] Univ Bonn, Helmholtz Inst Strahlen & Kernphys, D-53115 Bonn, Germany. [Barth, J.; Bieling, J.; Goertz, S.; Klein, F.; Panknin, R.; Pretz, J.; Windmolders, R.] Univ Bonn, Inst Phys, D-53115 Bonn, Germany. [Srnka, A.] AS CR, Inst Sci Instruments, Brno 61264, Czech Republic. [Dasgupta, S.; Sarkar, S.; Sinha, L.] Matrivani Inst Expt Res & Educ, Kolkata 700030, W Bengal, India. [Alexakhin, V. Y.; Alexeev, G. D.; Efremov, A.; Gavrichtchouk, O. P.; Gushterski, R.; Guskov, A.; Ivanshin, Y.; Kouznetsov, O.; Kroumchtein, Z. V.; Kuchinski, N.; Meshcheryakov, G.; Nagaytsev, I. A.; Olshevsky, A. G.; Rodionov, V.; Rossiyskaya, N. S.; Sapozhnikov, M. G.; Savin, I. A.; Shevchenko, O. Y.; Zemlyanichkina, E.; Zhuravlev, N.] Joint Inst Nucl Res, Dubna 141980, Moscow Region, Russia. [Adolph, C.; Braun, C.; Eyrich, W.; Lehmann, A.; Schmidt, A.] Univ Erlangen Nurnberg, Inst Phys, D-91054 Erlangen, Germany. [Buechele, M.; Fischer, H.; Guthoerl, T.; Heinsius, F. H.; Herrmann, F.; Koenigsmann, K.; Nerling, F.; Nowak, W. -D.; Schill, C.; Schmidt, K.; Schopferer, S.; Sirtl, S.; Ter Wolbeek, J.] Univ Freiburg, Inst Phys, D-79104 Freiburg, Germany. [Austregesilo, A.; Bicker, K.; von Hohenesche, N. du Fresne; Frolov, V.; Mallot, G. K.; Rocco, E.; Schoenning, K.; Schott, M.] CERN, CH-1211 Geneva 23, Switzerland. [Polak, J.; Sulc, M.] Tech Univ Liberec, Liberec 46117, Czech Republic. [Bordalo, P.; Franco, C.; Nunes, A. S.; Quaresma, M.; Quintans, C.; Ramos, S.; Silva, L.; Stolarski, M.] LIP, P-1000149 Lisbon, Portugal. [Bernhard, J.; von Hohenesche, N. du Fresne; von Harrach, D.; Jasinski, P.; Kabuss, E.; Kang, D.; Ostrick, M.; Pochodzalla, J.; Weisrock, T.; Wilfert, M.] Johannes Gutenberg Univ Mainz, Inst Kernphys, D-55099 Mainz, Germany. [Matsuda, T.] Miyazaki Univ, Miyazaki 8892192, Japan. [Alexandrov, Y.; Gerassimov, S.; Konorov, I.; Zavertyaev, M.] PN Lebedev Phys Inst, Moscow 119991, Russia. [Duennweber, W.; Faessler, M.; Geyer, R.; Schlueter, T.; Uman, I.] Univ Munich, Dept Phys, D-80799 Munich, Germany. [Austregesilo, A.; Bicker, K.; Chung, S. U.; Friedrich, J. M.; Gerassimov, S.; Grabmueller, S.; Grube, B.; Haas, F.; Hoeppner, C.; Huber, S.; Ketzer, B.; Konorov, I.; Kraemer, M.; Mann, A.; Nagel, T.; Neubert, S.; Paul, S.; Schmitt, L.; Uhl, S.] Tech Univ Munich, Dept Phys, D-85748 Garching, Germany. [Horikawa, N.] Nagoya Univ, Nagoya, Aichi 464, Japan. [Finger, M.; Finger, M., Jr.; Novy, J.] Charles Univ Prague, Fac Math & Phys, CR-18000 Prague, Czech Republic. [Jary, V.; Virius, M.] Czech Tech Univ, Prague 16636, Czech Republic. [Donskov, S. V.; Filin, A.; Khaustov, G. V.; Khokhlov, Y. A.; Kolosov, V. N.; Konstantinov, V. F.; Lednev, A. A.; Mikhailov, Y. V.; Nikolaenko, V. I.; Polyakov, V. A.; Ryabchikov, D. I.; Samoylenko, V. D.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino 142281, Russia. [Bedfer, Y.; Burtin, E.; Capozza, L.; Ferrero, A.; d'Hose, N.; Kouznetsov, O.; Kunne, F.; Magnon, A.; Makke, N.; Marchand, C.; Morreale, A.; Neyret, D.; Platchkov, S.; Thibaud, F.; Vandenbroucke, M.; Wollny, H.] CEA IRFU SPhN Saclay, F-91191 Gif Sur Yvette, France. [Lichtenstadt, J.] Tel Aviv Univ, Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Alekseev, M. G.; Birsa, R.; Bravar, A.; Cicuttin, A.; Crespo, M. L.; Dalla Torre, S.; Dasgupta, S. S.; Gobbo, B.; Sozzi, F.; Steiger, L.; Tessaro, S.; Tessarotto, F.] Ist Nazl Fis Nucl, Trieste Sect, I-34127 Trieste, Italy. [Bradamante, F.; Bressan, A.; Duic, V.; Elia, C.; Giorgi, M.; Levorato, S.; Makke, N.; Martin, A.; Polak, J.; Sbrizzai, G.; Schiavon, P.] Univ Trieste, Dept Phys, I-34127 Trieste, Italy. [Bradamante, F.; Bressan, A.; Duic, V.; Elia, C.; Giorgi, M.; Levorato, S.; Makke, N.; Martin, A.; Polak, J.; Sbrizzai, G.; Schiavon, P.] Univ Trieste, Ist Nazl Fis Nucl, Trieste Sect, I-34127 Trieste, Italy. [Cicuttin, A.; Crespo, M. L.] Abdus Salam Int Ctr Theoret Phys, I-34127 Trieste, Italy. [Amoroso, A.; Balestra, F.; Bertini, R.; Chiosso, M.; Garfagnini, R.; Gnesi, I.; Grasso, A.; Kotzinian, A. M.; Parsamyan, B.; Piragino, G.; Sosio, S.] Univ Turin, Dept Phys, I-10125 Turin, Italy. [Amoroso, A.; Balestra, F.; Bertini, R.; Chiosso, M.; Garfagnini, R.; Gnesi, I.; Grasso, A.; Kotzinian, A. M.; Parsamyan, B.; Piragino, G.; Sosio, S.] Univ Turin, Ist Nazl Fis Nucl, Torino Sect, I-10125 Turin, Italy. [Denisov, O. Y.; Maggiora, A.; Takekawa, S.] Ist Nazl Fis Nucl, Torino Sect, I-10125 Turin, Italy. [Panzieri, D.] Univ Piemonte Orientale, I-15100 Alessandria, Italy. [Klimaszewski, K.; Kurek, K.; Rondio, E.; Sandacz, A.; Sulej, R.; Sznajder, P.; Wislicki, W.] Natl Ctr Nucl Res, PL-00681 Warsaw, Poland. [Badelek, B.] Univ Warsaw, Fac Phys, PL-00681 Warsaw, Poland. [Dziewiecki, M.; Kurjata, R. P.; Marzec, J.; Zaremba, K.; Ziembicki, M.] Warsaw Univ Technol, Inst Radioelect, PL-00665 Warsaw, Poland. [Doshita, N.; Ishimoto, S.; Iwata, T.; Kondo, K.; Matsuda, H.; Michigami, T.; Miyachi, Y.; Suzuki, H.] Yamagata Univ, Yamagata 9928510, Japan. [Bordalo, P.; Ramos, S.; Schmidt, K.] Univ Tecn Lisboa, IST, P-1100 Lisbon, Portugal. [Chung, S. U.] Pusan Natl Univ, Dept Phys, Pusan 609735, South Korea. [Chung, S. U.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Horikawa, N.; Suzuki, H.] Chubu Univ, Kasugai, Aichi 4878501, Japan. [Ishimoto, S.] KEK, Tsukuba, Ibaraki 3050801, Japan. [Khokhlov, Y. A.] Moscow Inst Phys & Technol, Dolgoprudnyi 141700, Moscow Region, Russia. [Schmitt, L.] GSI mbH, D-64291 Darmstadt, Germany. RP Adolph, C (reprint author), Univ Erlangen Nurnberg, Inst Phys, D-91054 Erlangen, Germany. EM Andrea.Bressan@cern.ch RI Martin, Anna/I-9381-2012; Olshevskiy, Alexander/I-1580-2016; Kurjata, Robert/I-5112-2016; Levorato, Stefano/B-9582-2014; Srnka, A/E-2441-2012; Steiger, Lukas/H-3061-2014; Paul, Stephan/F-7596-2015; Paul, Stephan/K-9237-2016; Dasgupta, Shuddha Shankar/O-6118-2016; Friedrich, Jan/B-9024-2013; Koivuniemi, Jaakko/L-2959-2015; Zavertyaev, Mikhail/M-6844-2015; Gerassimov, Sergei/M-8779-2015 OI Austregesilo, Alexander/0000-0002-9291-4429; Amoroso, Antonio/0000-0002-3095-8610; Martin, Anna/0000-0002-1333-0143; Olshevskiy, Alexander/0000-0002-8902-1793; Kurjata, Robert/0000-0001-8547-910X; Levorato, Stefano/0000-0001-8067-5355; Steiger, Lukas/0000-0001-9772-9444; Paul, Stephan/0000-0002-8813-0437; Paul, Stephan/0000-0002-8813-0437; Friedrich, Jan/0000-0001-9298-7882; Koivuniemi, Jaakko/0000-0002-6817-5267; FU German Bundesministerium fur Bildung und Forschung; Czech Republic MEYS [ME492, LA242]; SAIL (CSR), Govt. of India; CERN-RFBR [08-02-91009, 12-02-91500]; Portuguese FCT-Fundacao para a Ciencia e Tecnologia; COMPETE; QREN [CERN/FP/109323/2009, CERN/FP/116376/2010, CERN/FP/123600/2011]; MEXT; JSPS [18002006, 20540299, 18540281]; Daiko Foundation; Yamada Foundation; DFG; EU [283286]; Israel Science Foundation; Polish NCN [DEC-2011/01/M/ST2/02350] FX Supported by the German Bundesministerium fur Bildung und Forschung.; Supported by Czech Republic MEYS Grants ME492 and LA242.; Supported by SAIL (CSR), Govt. of India.; Supported by CERN-RFBR Grants 08-02-91009 and 12-02-91500.; Supported by the Portuguese FCT-Fundacao para a Ciencia e Tecnologia, COMPETE and QREN, Grants CERN/FP/109323/2009, CERN/FP/116376/2010 and CERN/FP/123600/2011.; Supported by the MEXT and the JSPS under the Grants No. 18002006, No. 20540299 and No. 18540281; Daiko Foundation and Yamada Foundation; Supported by the DFG cluster of excellence 'Origin and Structure of the Universe' (www.universe-cluster.de); Supported by EU FP7 (HadronPhysics3, Grant Agreement number 283286); Supported by the Israel Science Foundation, founded by the Israel Academy of Sciences and Humanities; Supported by the Polish NCN Grant DEC-2011/01/M/ST2/02350 NR 12 TC 1 Z9 1 U1 0 U2 26 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 J9 EUR PHYS J C JI Eur. Phys. J. C PD OCT 9 PY 2013 VL 73 IS 10 AR 2581 DI 10.1140/epjc/s10052-013-2581-9 PG 9 WC Physics, Particles & Fields SC Physics GA 230QS UT WOS:000325357900001 ER PT J AU Akhmedov, EK Kopp, J AF Akhmedov, Evgeny Kh. Kopp, Joachim TI Neutrino oscillations: quantum mechanics vs. quantum field theory (vol 04, 008, 2010) SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Correction C1 [Akhmedov, Evgeny Kh.; Kopp, Joachim] Max Planck Inst Kernphys, D-69029 Heidelberg, Germany. [Akhmedov, Evgeny Kh.] Natl Res Ctr Kurchatov Inst, Moscow, Russia. [Kopp, Joachim] Fermilab Natl Accelerator Lab, Dept Theoret Phys, Batavia, IL 60510 USA. RP Akhmedov, EK (reprint author), Max Planck Inst Kernphys, Postfach 103980, D-69029 Heidelberg, Germany. EM akhmedov@mpi-hd.mpg.de; jkopp@fnal.gov NR 1 TC 2 Z9 2 U1 2 U2 5 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD OCT 9 PY 2013 IS 10 AR 052 DI 10.1007/JHEP10(2013)052 PG 3 WC Physics, Particles & Fields SC Physics GA 231PZ UT WOS:000325430900001 ER PT J AU Kassube, SA Fang, J Grob, P Yakovchuk, P Goodrich, JA Nogales, E AF Kassube, Susanne A. Fang, Jie Grob, Patricia Yakovchuk, Petro Goodrich, James A. Nogales, Eva TI Structural Insights into Transcriptional Repression by Noncoding RNAs That Bind to Human Pol II SO JOURNAL OF MOLECULAR BIOLOGY LA English DT Article DE transcription regulation; RNA polymerase II; electron microscopy; noncoding RNA; structure ID POLYMERASE-II; B2 RNA; ELECTRON-MICROSCOPY; ELONGATION COMPLEX; HEAT-SHOCK; ALU RNA; RESOLUTION; ARCHITECTURE; VISUALIZATION; INITIATION AB Gene transcription is regulated in response to environmental changes and developmental cues. In mammalian cells subjected to stress conditions such as heat shock, transcription of most protein-coding genes decreases, while the transcription of heat shock protein genes increases. Repression involves direct binding to RNA polymerase II (Pol II) of certain noncoding RNAs (ncRNAs) that are upregulated upon heat shock. Another class of ncRNAs is also upregulated and binds to Pol II but does not inhibit transcription. Incorporation of repressive ncRNAs into pre-initiation complexes prevents transcription initiation, while non-repressive ncRNAs are displaced from Pol II by TFIIF. Here, we present cryo-electron microscopy reconstructions of human Pol H in complex with six different ncRNAs from mouse and human. Our structures show that both repressive and non-repressive ncRNAs bind to a conserved binding site within the cleft of Pol II. The site, which is also shared with a previously characterized yeast aptamer, is close to the active center and, thus, in an ideal position to regulate transcription. Importantly, additional RNA elements extend flexibly beyond the docking site. We propose that the differences concerning the repressive activity of the ncRNAs analyzed must be due to the distinct character of these more unstructured, flexible segments of the RNA that emanate from the cleft. (c) 2012 Elsevier Ltd. All rights reserved. C1 [Kassube, Susanne A.] Univ Calif Berkeley, Biophys Grad Grp, Berkeley, CA 94720 USA. [Fang, Jie; Grob, Patricia; Nogales, Eva] Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA. [Yakovchuk, Petro; Goodrich, James A.] Univ Colorado, Dept Chem & Biochem, Boulder, CO 80309 USA. [Nogales, Eva] Univ Calif Berkeley, Mol & Cell Biol Dept, Berkeley, CA 94720 USA. [Nogales, Eva] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. RP Nogales, E (reprint author), Univ Calif Berkeley, 708C Stanley Hall, Berkeley, CA 94720 USA. EM enogales@lbl.gov FU Boehringer Ingelheim Fonds; National Institute of General Medical Sciences [GM63072, GM068414] FX We thank M. Jinek for comments on the manuscript. S.K. acknowledges a fellowship from the Boehringer Ingelheim Fonds. The work was supported by National Institute of General Medical Sciences grants GM63072 (E.N.) and GM068414 (J.A.G.). E.N. is a Howard Hughes Medical Institute investigator. NR 31 TC 6 Z9 8 U1 2 U2 26 PU ACADEMIC PRESS LTD- ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL RD, LONDON NW1 7DX, ENGLAND SN 0022-2836 J9 J MOL BIOL JI J. Mol. Biol. PD OCT 9 PY 2013 VL 425 IS 19 BP 3639 EP 3648 DI 10.1016/j.jmb.2012.08.024 PG 10 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA 226MP UT WOS:000325040800006 PM 22954660 ER PT J AU Novikova, IV Hennelly, SP Tung, CS Sanbonmatsu, KY AF Novikova, Irina V. Hennelly, Scott P. Tung, Chang-Shung Sanbonmatsu, Karissa Y. TI Rise of the RNA Machines: Exploring the Structure of Long Non-Coding RNAs SO JOURNAL OF MOLECULAR BIOLOGY LA English DT Review DE long non-coding RNA; lncRNA; lincRNA; lncRNA structure; epigenetics ID SAM-I RIBOSWITCH; X-CHROMOSOME INACTIVATION; CONTROLS GENE-EXPRESSION; SECONDARY STRUCTURE; S-ADENOSYLMETHIONINE; CRYSTAL-STRUCTURE; NUCLEAR PARASPECKLES; STRUCTURE PREDICTION; ANGSTROM RESOLUTION; LINEAGE COMMITMENT AB Novel, profound and unexpected roles of long non-coding RNAs (lncRNAs) are emerging in critical aspects of gene regulation. Thousands of lncRNAs have been recently discovered in a wide range of mammalian systems, related to development, epigenetics, cancer, brain function and hereditary disease. The structural biology of these lncRNAs presents a brave new RNA world, which may contain a diverse zoo of new architectures and mechanisms. While structural studies of lncRNAs are in their infancy, we describe existing structural data for lncRNAs, as well as crystallographic studies of other RNA machines and their implications for lncRNAs. We also discuss the importance of dynamics in RNA machine mechanism. Determining commonalities between lncRNA systems will help elucidate the evolution and mechanistic role of lncRNAs in disease, creating a structural framework necessary to pursue lncRNA-based therapeutics. Published by Elsevier Ltd. C1 [Novikova, Irina V.; Hennelly, Scott P.; Tung, Chang-Shung; Sanbonmatsu, Karissa Y.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Sanbonmatsu, KY (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM kys@lanl.gov FU US Department of Energy via Los Alamos National Laboratory, Laboratory Directed Research and Development FX The work was performed under the auspices of the US Department of Energy via Los Alamos National Laboratory, Laboratory Directed Research and Development. NR 135 TC 34 Z9 37 U1 7 U2 124 PU ACADEMIC PRESS LTD- ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL RD, LONDON NW1 7DX, ENGLAND SN 0022-2836 J9 J MOL BIOL JI J. Mol. Biol. PD OCT 9 PY 2013 VL 425 IS 19 BP 3731 EP 3746 DI 10.1016/j.jmb.2013.02.030 PG 16 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA 226MP UT WOS:000325040800013 PM 23467124 ER PT J AU Zhang, W Morton, SA Wong, PKJ Lu, B Xu, YB de Jong, MP van der Wiel, WG van der Laan, G AF Zhang, Wen Morton, Simon A. Wong, P. K. Johnny Lu, Bin Xu, Yongbing de Jong, Michel P. van der Wiel, Wilfred G. van der Laan, Gerrit TI Microscopic origin of the reduced magnetocrystalline anisotropy with increasing oxide content in Co80Pt20 : oxide thin films SO JOURNAL OF PHYSICS D-APPLIED PHYSICS LA English DT Article ID MAGNETIC-CIRCULAR-DICHROISM; ASSEMBLED CO CLUSTERS; X-RAY DICHROISM; PERPENDICULAR MEDIA; ORBITAL MAGNETIZATION; TRANSITION-METALS; MOMENT; COBALT; 3D; CRYSTALS AB Angle-dependent x-ray magnetic circular dichroism at the Co L-2.3 edges has been utilized to systematically study Co80Pt20 : WO3 perpendicular magnetic recording thin films, in which the magnetocrystalline anisotropy significantly drops as the oxide volume fraction increases. The microscopic origin of this phenomenon in the studied films can be mainly attributed to an increase in orbital moment normal to the grain-oxide interface, with increasing oxide volume fraction, which arises from a more pronounced effect of symmetry breaking at the grain-oxide interface in smaller grains. C1 [Zhang, Wen; Wong, P. K. Johnny; de Jong, Michel P.; van der Wiel, Wilfred G.] Univ Twente, MESA Inst Nanotechnol, NanoElect Grp, NL-7500 AE Enschede, Netherlands. [Zhang, Wen; Xu, Yongbing] Univ York, Dept Elect, Spintron & Nanodevices Lab, York YO10 5DD, N Yorkshire, England. [Morton, Simon A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Lu, Bin] Seagate Technol, Fremont, CA 94538 USA. [van der Laan, Gerrit] Magnet Spect Grp, Diamond Light Source, Didcot OX11 0DE, Oxon, England. RP Zhang, W (reprint author), Southeast Univ, Dept Phys, Nanjing 211189, Jiangsu, Peoples R China. EM xiaotur@gmail.com RI van der Wiel, Wilfred/F-8812-2014; Wong, Johnny/G-1745-2010; van der Laan, Gerrit/Q-1662-2015 OI van der Wiel, Wilfred/0000-0002-3479-8853; Wong, Johnny/0000-0003-4645-0384; van der Laan, Gerrit/0000-0001-6852-2495 FU Office of Science, Office of Basic Energy Sciences, of the US Department of Energy [DE-AC02-05CH11231] FX The authors would like to thank Dr Elke Arenholz and Dr Catherine Jenkins for their kind support at BL 6.3.1. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the US Department of Energy under Contract No DE-AC02-05CH11231. NR 53 TC 2 Z9 2 U1 1 U2 11 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0022-3727 J9 J PHYS D APPL PHYS JI J. Phys. D-Appl. Phys. PD OCT 9 PY 2013 VL 46 IS 40 AR 405001 DI 10.1088/0022-3727/46/40/405001 PG 5 WC Physics, Applied SC Physics GA 224DC UT WOS:000324861100011 ER PT J AU Brake, MR Segalman, DJ AF Brake, M. R. Segalman, D. J. TI Modelling localized nonlinearities in continuous systems via the method of augmentation by non-smooth basis functions SO PROCEEDINGS OF THE ROYAL SOCIETY A-MATHEMATICAL PHYSICAL AND ENGINEERING SCIENCES LA English DT Article DE vibration; nonlinear constraints; continuous systems; non-smooth basis functions; model reduction; localized nonlinearities ID IMPACT RESPONSE; BEAM SYSTEM; DYNAMICS; VIBRATION; BIFURCATIONS; CONSTRAINTS; REDUCTION; FRICTION; FLUID; FLOW AB Existing solutions for continuous systems with localized, non-smooth nonlinearities (such as impacts) focus on exact methods for satisfying the nonlinear constitutive equations. Exact methods often require that the non-smooth nonlinearities be expressed as piecewise-linear functions, which results in a series of mapping equations between each linear regime of the nonlinearities. This necessitates exact transition times between each linear regime of the nonlinearities, significantly increasing computational time, and limits the analysis to only considering a small number of nonlinearities. A new method is proposed in which the exact, nonlinear constitutive equations are satisfied by augmenting the system's primary basis functions with a set of non-smooth basis functions. Two consequences are that precise contact times are not needed, enabling greater computational efficiency than exact methods, and localized nonlinearities are not limited to piecewise-linear functions. Since each nonlinearity requires only a few non-smooth basis functions, this method is easily expanded to handle large numbers of nonlinearities throughout the domain. To illustrate the application of this method, a pinned-pinned beam example is presented. Results demonstrate that this method requires significantly fewer basis functions to achieve convergence, compared with linear and exact methods, and that this method is orders of magnitude faster than exact methods. C1 [Brake, M. R.; Segalman, D. J.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Brake, MR (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM mrbrake@sandia.gov FU US Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporations, for the US Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL85000. NR 35 TC 1 Z9 1 U1 0 U2 5 PU ROYAL SOC PI LONDON PA 6-9 CARLTON HOUSE TERRACE, LONDON SW1Y 5AG, ENGLAND SN 1364-5021 EI 1471-2946 J9 P ROY SOC A-MATH PHY JI Proc. R. Soc. A-Math. Phys. Eng. Sci. PD OCT 8 PY 2013 VL 469 IS 2158 AR 20130260 DI 10.1098/rspa.2013.0260 PG 20 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 298IU UT WOS:000330318200009 ER PT J AU Bleichert, F Balasov, M Chesnokov, I Nogales, E Botchan, MR Berger, JM AF Bleichert, Franziska Balasov, Maxim Chesnokov, Igor Nogales, Eva Botchan, Michael R. Berger, James M. TI A Meier-Gorlin syndrome mutation in a conserved C-terminal helix of Orc6 impedes origin recognition complex formation SO ELIFE LA English DT Article ID PRE-REPLICATIVE COMPLEXES; PARTICLE ELECTRON CRYOMICROSCOPY; MULTIPLE SEQUENCE ALIGNMENT; DNA-REPLICATION; PRIMORDIAL DWARFISM; SACCHAROMYCES-CEREVISIAE; CONFORMATIONAL-CHANGES; FUNCTIONAL-ANALYSIS; ATP-HYDROLYSIS; PROTEIN AB In eukaryotes, DNA replication requires the origin recognition complex (ORC), a six-subunit assembly that promotes replisome formation on chromosomal origins. Despite extant homology between certain subunits, the degree of structural and organizational overlap between budding yeast and metazoan ORC has been unclear. Using 3D electron microscopy, we determined the subunit organization of metazoan ORC, revealing that it adopts a global architecture very similar to the budding yeast complex. Bioinformatic analysis extends this conservation to Orc6, a subunit of somewhat enigmatic function. Unexpectedly, a mutation in the Orc6 C-terminus linked to Meier-Gorlin syndrome, a dwarfism disorder, impedes proper recruitment of Orc6 into ORC; biochemical studies reveal that this region of Orc6 associates with a previously uncharacterized domain of Orc3 and is required for ORC function and MCM2-7 loading in vivo. Together, our results suggest that Meier-Gorlin syndrome mutations in Orc6 impair the formation of ORC hexamers, interfering with appropriate ORC functions. C1 [Bleichert, Franziska] Univ Calif Berkeley, Miller Inst Basic Res Sci, Berkeley, CA 94720 USA. [Bleichert, Franziska; Nogales, Eva; Botchan, Michael R.; Berger, James M.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Balasov, Maxim; Chesnokov, Igor] Univ Alabama Birmingham, Med Sch Birmingham, Dept Biochem & Mol Genet, Birmingham, AL USA. [Nogales, Eva] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. [Nogales, Eva] Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA. RP Botchan, MR (reprint author), Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA. EM mbotchan@berkeley.edu; jmberger@jhmi.edu FU National Institutes of Health [GM071747, R37 30490, GM097052]; Howard Hughes Medical Institute; Miller Institute for Basic Research in Science FX National Institutes of Health GM071747 James M Berger; Howard Hughes Medical Institute Eva Nogales; Miller Institute for Basic Research in Science Franziska Bleichert; National Institutes of Health R37 30490 Michael R Botchan; National Institutes of Health GM097052 Igor Chesnokov NR 84 TC 13 Z9 13 U1 0 U2 3 PU ELIFE SCIENCES PUBLICATIONS LTD PI CAMBRIDGE PA SHERATON HOUSE, CASTLE PARK, CAMBRIDGE, CB3 0AX, ENGLAND SN 2050-084X J9 ELIFE JI eLife PD OCT 8 PY 2013 VL 2 AR e00882 DI 10.7554/eLife.00882 PG 29 WC Biology SC Life Sciences & Biomedicine - Other Topics GA 274WI UT WOS:000328636500002 PM 24137536 ER PT J AU Nellas, RB Johnson, QR Shen, TY AF Nellas, Ricky B. Johnson, Quentin R. Shen, Tongye TI Solvent-Induced alpha- to 3(10)-Helix Transition of an Amphiphilic Peptide SO BIOCHEMISTRY LA English DT Article ID ALPHA,ALPHA-DIALKYL AMINO-ACIDS; PSEUDOMONAS-AERUGINOSA LST-03; APOLIPOPROTEIN-A-I; AMINOISOBUTYRIC-ACID; SECONDARY STRUCTURE; CRYSTAL-STRUCTURE; PARALLEL PACKING; STABLE LIPASE; HELIX; PROTEINS AB The amphiphilic peptide of the triacylglycerol lipase derived from Pseudomonas aeruginosa plays a critical role in guarding the gate for ligand access. Conformations of this peptide at several water-oil interfaces and in protein environments were compared using atomistic simulations with explicit solvents. In oil-containing solvents, this peptide is able to retain a folded structure. Interestingly, when the peptide is immersed in a low-polarity solvent environment, it exhibits a "coalesced" helix structure, which has both alpha- and 3(10)-helix components. The observation that the 3(10)-helical conformation is populated in a highly nonpolar environment is consistent with a previous report on polymethylalanine. Frequent interconversions of the secondary structure (between alpha-helix and 3(10)-helix) of the peptide are also observed. We further studied how this solvent-induced structural transition may be connected to the trigger mechanism of lipase gating and how the lipase senses the hydrophobic-hydrophilic interface. C1 [Nellas, Ricky B.; Shen, Tongye] Univ Tennessee, Dept Biochem & Cellular & Mol Biol, Knoxville, TN 37996 USA. [Nellas, Ricky B.; Johnson, Quentin R.; Shen, Tongye] Univ Tennessee, Oak Ridge Natl Lab, Ctr Biophys Mol, Oak Ridge, TN 37830 USA. [Johnson, Quentin R.] Univ Tennessee, Oak Ridge Natl Lab, Grad Sch Genome Sci & Technol, Knoxville, TN 37996 USA. RP Shen, TY (reprint author), Univ Tennessee, Dept Biochem & Cellular & Mol Biol, Knoxville, TN 37996 USA. EM tshen@utk.edu RI Shen, Tongye/A-9718-2008 OI Shen, Tongye/0000-0003-1495-3104 FU Petroleum Research Fund [52616-DNI6]; National Science Foundation FX Financial support from the Petroleum Research Fund administered by the American Chemical Society (52616-DNI6) is gratefully acknowledged. Q.R.J. is supported by National Science Foundation-funded graduate fellowship program SCALE-IT. NR 53 TC 5 Z9 5 U1 0 U2 8 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0006-2960 EI 1943-295X J9 BIOCHEMISTRY-US JI Biochemistry PD OCT 8 PY 2013 VL 52 IS 40 BP 7137 EP 7144 DI 10.1021/bi400537z PG 8 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA 243YY UT WOS:000326355500021 PM 24066804 ER PT J AU Lascola, R Knight, DA Mohtadi, R Sivasubramanian, P Zidan, R AF Lascola, Robert Knight, Douglas A. Mohtadi, Rana Sivasubramanian, PremKurnar Zidan, Ragaiy TI Synthesis and structural characterization of stabilized aluminum borohydride adducts with triethylenediamine SO INTERNATIONAL JOURNAL OF HYDROGEN ENERGY LA English DT Article DE Hydrogen storage; Metal hydrides; Aluminum borohydride; Adduction; Raman spectroscopy ID HYDROGEN STORAGE; TRIMETHYLAMINE-BORANE; MOLECULAR-STRUCTURE; METAL BOROHYDRIDES; CRYSTAL-STRUCTURE; SOLID HYDROGEN; RAMAN-SPECTRA; TETRAHYDROBORATE; DIBORANE; COMPLEX AB The 1:1 and 1:2 adducts of aluminum borohydride (Al(BH4)(3)) and the Lewis base triethylenediamine (TEDA) and their thermal decomposition products were synthesized and structurally characterized by Raman spectroscopy, X-ray diffraction, and thermogravimetric analysis. Both adducts are more stable than Al(BH4)(3) with respect to thermal decomposition and release of diborane. The structural analysis indicates that stabilization occurs through the donation of electron density through the N-Al dipolar bonds, leading to a more ionic character of the borohydride subunit. The 1:2 adduct, which has more electron donation, shows more ionic character and greater stability. For both adducts, the displaced borohydride group forms a dipolar bond with the second N lone pair of the TEDA, preserving much of the H content of the material. Decomposition occurs by internal rearrangement of borohydride, forming 1:1 and 1:2 TEDA center dot BH3 adducts, followed by release of H-2 from the Al bonding center. The relative stability of the adducts encourages continuing exploration of Lewis base-stabilized borohydrides as an improved hydrogen storage material. Copyright (C) 2013, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved. C1 [Lascola, Robert] Savannah River Natl Lab, Sci & Technol Directorate, Aiken, SC 29808 USA. [Knight, Douglas A.; Zidan, Ragaiy] Savannah River Natl Lab, Clean Energy Directorate, Aiken, SC 29808 USA. [Mohtadi, Rana; Sivasubramanian, PremKurnar] Toyota Res Inst North Amer, Mat Res Dept, Ann Arbor, MI 48105 USA. RP Zidan, R (reprint author), Savannah River Natl Lab, Clean Energy Directorate, POB A, Aiken, SC 29808 USA. EM Ragaiy.Zidan@srnl.doe.gov OI Lascola, Robert/0000-0002-6784-5644; Knight, David/0000-0001-5510-6265 FU Toyota Research Institute of North America; U.S. Department of Energy [DE-AC09-08SR22470] FX R.L., D.A.K, and R.Z. would like to thank: the Toyota Research Institute of North America for financial support through a Cooperative Research and Development Agreement, Dr. Patrick O'Rourke and Mr. David Missimer (SRNL) for assistance with XRD measurements, and Mr. Joseph Wheeler (SRNL) for assistance with laboratory operations. This manuscript has been authored by Savannah River Nuclear Solutions, LLC under Contract No. DE-AC09-08SR22470 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting this article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this work, or allow others to do so, for United States Government purposes. NR 44 TC 4 Z9 4 U1 3 U2 22 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-3199 EI 1879-3487 J9 INT J HYDROGEN ENERG JI Int. J. Hydrog. Energy PD OCT 8 PY 2013 VL 38 IS 30 BP 13368 EP 13380 DI 10.1016/j.ijhydene.2013.07.100 PG 13 WC Chemistry, Physical; Electrochemistry; Energy & Fuels SC Chemistry; Electrochemistry; Energy & Fuels GA 242CE UT WOS:000326214200027 ER PT J AU Kim, DS Fujimoto, CH Hibbs, MR Labouriau, A Choe, YK Kim, YS AF Kim, Dae Sik Fujimoto, Cy H. Hibbs, Michael R. Labouriau, Andrea Choe, Yoong-Kee Kim, Yu Seung TI Resonance Stabilized Perfluorinated lonomers for Alkaline Membrane Fuel Cells SO MACROMOLECULES LA English DT Article ID ANION-EXCHANGE MEMBRANES; POLYMER ELECTROLYTE; OXYGEN REDUCTION; INTERFACE; PERFORMANCE; CATALYST; PEFCS; POLYAROMATICS; SPECTROSCOPY; DURABILITY AB Perfluorosulfonic acids such as Nafion are industrial standard cation exchange ionomers for polymer electrolyte membrane fuel cells because of their high gas permeability, hydrophobicity, and inertness to electro-chemical reaction. In this research, pentamethylguanidinium functionalized, perfluorinated hydroxide conducting ionomers for alkaline membrane fuel cells were prepared and characterized. The alkaline stability of the ionomers largely depended on the adjacent group that connected the cation; Sulfone guanidinium functionalized ionomer degraded almost completely after soaking in 0.5 M NaOH at 80 degrees C for 24 h, while phenylguanidinium functionalized ionomer did not degrade under the same conditions for 72 h. Spectroscopic data and density functional theory calculation suggested that the stability of the phenylguanidinium ionomer was greatly improved by charge delocalization of the formed resonance structure. Alkaline membrane fuel cells using the resonance stabilized perfluorinated ionomer in the catalyst layers on quaternized polyphenylene membrane showed excellent performance (ca. maximum power density = 466 mW/cm(2)) and promising stability (ca. Tafel slope degradation rate = 225 mu V/dec h) at 80 degrees C under H-2/air conditions. C1 [Kim, Dae Sik; Kim, Yu Seung] Los Alamos Natl Lab, Sensors & Electrochem Devices Grp, Los Alamos, NM 87545 USA. [Fujimoto, Cy H.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Hibbs, Michael R.] Sandia Natl Labs, Mat Devices & Energy Technol Grp, Albuquerque, NM 87185 USA. [Labouriau, Andrea] Los Alamos Natl Lab, Polymers & Coatings Grp, Los Alamos, NM 87545 USA. [Choe, Yoong-Kee] Natl Inst Adv Ind Sci & Technol, Tsukuba, Ibaraki 3058575, Japan. RP Kim, YS (reprint author), Los Alamos Natl Lab, Sensors & Electrochem Devices Grp, POB 1663, Los Alamos, NM 87545 USA. EM yskim@lanl.gov RI Choe, Yoong-Kee/A-9635-2008 FU US Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; US DOE; Ministry of Economy, Trade and Industry of Japan through Japan US cooperation on clean energy technology program FX This work was supported by the US Department of Energy at Los Alamos National Laboratory operated by Los Alamos National Security LLC under Contract DE-AC52-06NA25396. Sandia National Laboratory is a multiprogram laboratory operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Company, for the U.S. Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL85000. The authors also thank US DOE Fuel Cell Technologies Program, Technology Development Manager Dr. Nancy Garland, for financial support. Y.-K.C acknowledges financial support from the Ministry of Economy, Trade and Industry of Japan through Japan US cooperation on clean energy technology program. NR 58 TC 30 Z9 30 U1 4 U2 105 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD OCT 8 PY 2013 VL 46 IS 19 BP 7826 EP 7833 DI 10.1021/ma401568f PG 8 WC Polymer Science SC Polymer Science GA 243YV UT WOS:000326355200027 ER PT J AU Akgun, B Satija, S Nanda, H Pirrone, GF Shi, XM Engen, JR Kent, MS AF Akgun, Bulent Satija, Sushi Nanda, Hirsh Pirrone, Gregory F. Shi, Xiaomeng Engen, John R. Kent, Michael S. TI Conformational Transition of Membrane-Associated Terminally Acylated HIV-1 Nef SO STRUCTURE LA English DT Article ID VIRUS TYPE-1 NEF; BILAYER-LIPID MEMBRANES; CRYSTAL-STRUCTURE; SH3 DOMAIN; VIRAL INFECTIVITY; N-MYRISTOYLATION; STRUCTURAL BASIS; DOWN-REGULATION; PROTEIN-KINASE; I NEF AB Many proteins are posttranslationally modified by acylation targeting them to lipid membranes. While methods such as X-ray crystallography and nuclear magnetic resonance are available to determine the structure of folded proteins in solution, the precise position of folded domains relative to a membrane remains largely unknown. We used neutron and X-ray reflection methods to measure the displacement of the core domain of HIV Nef from lipid membranes upon insertion of the N-terminal myristate.HIV-1 accessory proteins, progression. Upon insertion of the myristate and residues from the N-terminal arm, Nef transitions from a closed-to-open conformation that positions the core domain 70 A from the lipid headgroups. This work rules out previous speculation that the Nef core remains closely associated with the membrane to optimize interactions with the cytoplasmic domain of MHC-1. C1 [Akgun, Bulent; Satija, Sushi; Nanda, Hirsh] NIST, Gaithersburg, MD 20899 USA. [Akgun, Bulent; Nanda, Hirsh] Univ Maryland, Dept Mat Sci & Engn, College Pk, MD 20742 USA. [Akgun, Bulent] Bogazici Univ, Dept Chem, TR-34342 Istanbul, Turkey. [Pirrone, Gregory F.; Shi, Xiaomeng; Engen, John R.] Northeastern Univ, Dept Chem & Chem Biol, Boston, MA 02115 USA. [Kent, Michael S.] Sandia Natl Labs, Albuquerque, NM 87123 USA. RP Kent, MS (reprint author), Sandia Natl Labs, Albuquerque, NM 87123 USA. EM mskent@sandia.gov RI Akgun, Bulent/H-3798-2011 FU Sandia Corporation, a Lockheed Martin Company, for the U.S. Department of Energy [DE-AC04-94AL85000]; National Institute of Standards and Technology, the U.S. Department of Commerce; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; NIH [R01-GM086507, R01-GM101647-02] FX Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the U.S. Department of Energy under contract DE-AC04-94AL85000. We acknowledge the support of the National Institute of Standards and Technology, the U.S. Department of Commerce, in providing the neutron research facilities used in this work. Research conducted at ORNL's Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. This work was supported by NIH grant R01-GM086507 (to M.S.K. and J.R.E.) and R01-GM101647-02 (to H.N.) Commercial materials, instruments, and equipment are identified in this paper to specify the experimental procedure as completely as possible. In no case does such identification imply a recommendation or endorsement by the National Institute of Standards and Technology, nor does it imply that the materials, instruments, or equipment identified are necessarily the best available for the purpose. NR 54 TC 9 Z9 9 U1 2 U2 18 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0969-2126 EI 1878-4186 J9 STRUCTURE JI Structure PD OCT 8 PY 2013 VL 21 IS 10 BP 1822 EP 1833 DI 10.1016/j.str.2013.08.008 PG 12 WC Biochemistry & Molecular Biology; Biophysics; Cell Biology SC Biochemistry & Molecular Biology; Biophysics; Cell Biology GA 244TQ UT WOS:000326413500013 PM 24035710 ER PT J AU Aad, G Abajyan, T Abbott, B Abdallah, J Khalek, SA Abdelalim, AA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Addy, TN Adelman, J Adomeit, S Adye, T Aefsky, S Aguilar-Saavedra, JA Agustoni, M Ahlen, SP Ahles, F Ahmad, A Ahsan, M Aielli, G Akesson, TPA Akimoto, G Akimov, AV Alam, MA Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alessandria, F Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Aliev, M Alimonti, G Alison, J Allbrooke, BMM Allison, LJ Allport, PP Allwood-Spiers, SE Almond, J Aloisio, A Alon, R Alonso, A Alonso, F Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Coutinho, YA Amelung, C Ammosov, VV dos Santos, SPA Amorim, A Amoroso, S Amram, N Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Anduaga, XS Angelidakis, S Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonaki, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Apolle, R Arabidze, G Aracena, I Arai, Y Arce, ATH Arfaoui, S Arguin, JF Argyropoulos, S Arik, E Arik, M Armbruster, AJ Arnaez, O Arnal, V Artamonov, A Artoni, G Arutinov, D Asai, S Asbah, N Ask, S Aring;sman, B Asquith, L Assamagan, K Astalos, R Astbury, A Atkinson, M Auerbach, B Auge, E Augsten, K Aurousseau, M Avolio, G Axen, D Azuelos, G Azuma, Y Baak, MA Bacci, C Bach, AM Bachacou, H Bachas, K Backes, M Backhaus, M Mayes, JB Badescu, E Bagiacchi, P Bagnaia, P Bai, Y Bailey, DC Bain, T Baines, JT Baker, OK Baker, S Balek, P Balli, F Banas, E Banerjee, P Banerjee, S Fi, DB Bangert, A Bansal, V Bansil, HS Barak, L Baranov, SP Barber, T Barberio, EL Barberis, D Barbero, M Bardin, DY Barillari, T Barisonzi, M Barklow, T Barlow, N Barnett, BM Barnett, RM Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartsch, V Basye, A Bates, RL Batkova, L Batley, JR Battaglia, A Battistin, M Bauer, F Bawa, HS Beale, S Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, S Beckingham, M Becks, KH Beddall, AJ Beddall, A Bedikian, S Bednyakov, VA Bee, CP Beemster, LJ Beermann, TA Begel, M Belanger-Champagne, C Bell, PJ Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belloni, A Beloborodova, OL Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Benslama, K Bentvelsen, S Berge, D Kuutmann, EB Berger, N Berghaus, F Berglund, E Beringer, J Bernat, P Bernhard, R Bernius, C 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Zibell, A. Zieminska, D. Zimin, N. I. Zimmermann, C. Zimmermann, R. Zimmermann, S. Zimmermann, S. Zinonos, Z. Ziolkowski, M. Zitoun, R. Zivkovic, L. Zmouchko, V. V. Zobernig, G. Zoccoli, A. Nedden, M. Zur Zutshi, V. Zwalinski, L. CA ATLAS Collaboration TI Measurement of the differential cross-section of B+ meson production in pp collisions at root s=7 TeV at ATLAS SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering ID BOTTOM-QUARK PRODUCTION; PROTON-PROTON COLLISIONS; P(P)OVER-BAR COLLISIONS; HADRONIC COLLISIONS; JET FRAGMENTATION; HEAVY QUARKS; MODEL; DETECTOR; DECAYS; MUON AB The production cross-section of B+ mesons is measured as a function of transverse momentum p T and rapidity y in proton-proton collisions at centre-of-mass energy root s = 7 TeV, using 2.4 fb(-1) of data recorded with the ATLAS detector at the Large Hadron Collider. 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[Alexa, C.; Badescu, E.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Cuciuc, C. -M.; Dinut, F.; Dita, P.; Dita, S.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. [Darlea, G. L.] Univ Politehn Bucuresti, Bucharest, Romania. [Stoicea, G.] West Univ Timisoara, Timisoara, Romania. [Silva, M. L. Gonzalez; Garzon, G. Otero Y.; Piegaia, R.; Romeo, G.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Ask, S.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Buttinger, W.; Carter, J. R.; Chapman, J. D.; French, S. T.; Frost, J. A.; Gillam, T. P. S.; Hill, J. C.; Hsu, P. J.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Moeller, V.; Mueller, T.; Parker, M. A.; Robinson, D.; Sandoval, T.; Thomson, M.; Ward, C. P.; Williams, S.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Koffas, T.; Lacey, J.; Marchand, J. F.; McCarthy, T. G.; Oakham, F. G.; Randrianarivony, K.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Anastopoulos, C.; Andari, N.; Anghinolfi, F.; Avolio, G.; Baak, M. A.; Fi, D. Ban; Battistin, M.; Bellomo, M.; Beltramello, O.; Berge, D.; Bogaerts, J. A.; Boyd, J.; Bremer, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Catmore, J. R.; Cattai, A.; Barajas, C. A. Chavez; Childers, J. T.; Chromek-Burckhart, D.; Cote, D.; Danielsson, H. O.; Dell'Acqua, A.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dopke, J.; Dudarev, A.; Uhrssen, M. D.; Ellis, N.; Elsing, M.; Fabre, C.; Facini, G.; Farthouat, P.; Fassnacht, P.; Franchino, S.; Francis, D.; Franz, S.; Froidevaux, D.; Gabaldon, C.; Garonne, V.; Gianotti, F.; Gillberg, D.; Godlewski, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Haas, S.; Hauschild, M.; Hawkings, R. J.; Heller, M.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Hubacek, Z.; Huhtinen, M.; Jaekel, M. R.; Jansen, H.; Jenni, P.; Jungst, R. M.; Kaneda, M.; Klioutchnikova, T.; Oneke, K. K.; Lantzsch, K.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mapelli, L.; Martin, B.; Messina, A.; Meyer, J.; Michal, S.; Molfetas, A.; Morley, A. K.; Mornacchi, G.; Muenstermann, D.; Nairz, A. M.; Nakahama, Y.; Negri, G.; Nessiad, M.; Nicquevert, B.; Nordberg, M.; Ohm, C. C.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Petersen, J.; Pommes, K.; Poppleton, A.; Poulard, G.; Prasad, S.; Raymond, M.; Rembser, C.; Dos Santos, D. Roda; Roe, S.; Salek, D.; Salzburger, A.; Savu, D. O.; Schlenker, S.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Spiwoks, R.; Stewart, G. A.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; Van der Ster, D.; Van Eldik, N.; Vandelli, W.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Winklmeier, F.; Wotschack, J.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Boveia, A.; Canelli, F.; Cheng, Y.; Choudalakis, G.; Fiascaris, M.; Gardner, R. W.; Plante, I. Jen-La; Kapliy, A.; Li, H. L.; Meehan, S.; Melachrinos, C.; Merritt, F. S.; Meyer, C.; Miller, D. W.; Okumura, Y.; Onyisiaf, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Shochet, M. J.; Tompkins, L.; Tuggle, J. M.; Vukotic, I.; Webster, J. S.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Cottin, G.; Diaz, M. A.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Carquin, E.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lu, F.; Ouyang, Q.; Shan, L. Y.; Wang, J.; Xu, D.; Yao, L.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Chen, S.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Feng, C.; Ge, P.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Yang, H.] Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200030, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Clermont Univ, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] CNRS, IN2P3, Clermont Ferrand, France. [Ahmad, A.; Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Chen, Y.; Dodd, J.; Guo, J.; Hu, D.; Hughes, E. W.; Nikiforou, N.; Parsons, J. A.; Penson, A.; Reale, V. Perez; Scherzer, M. I.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Williams, E.; Willis, W.; Wulf, E.; Zivkovic, L.] Columbia Univ, Nevis Lab, Columbia, NY USA. [Alonso, A.; Boelaert, N.; Dam, M.; Gregersen, K.; Hansen, J. R.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Heisterkamp, S.; Jakobsen, S.; Jez, P.; Joergensen, M. D.; Kadlecik, P.; Klinkby, E. B.; Loevschall-Jensen, A. E.; Lundquist, J.; Mackeprang, R.; Mehlhase, S.; Monk, J.; Petersen, T. C.; Pingel, A.; Simonyan, M.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] INFN Grp Collegato Cosenza, Arcavacata Di Rende, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; Blocki, J.; de Renstrom, P. A. Bruckman; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Malecki, P.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Turala, M.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.; Zemla, A.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Ahmad, A.; Cao, T.; Yagci, K. Dindar; Firan, A.; Hoffman, J.; Joffe, D.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Rios, R. R.; Sekula, S. J.; Stroynowski, R.; Wang, H.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Ahsan, M.; Izen, J. M.; Lou, X.; Namasivayam, H.; Reeves, K.; Wong, W. C.] Univ Texas Dallas, Dept Phys, Dallas, TX 75230 USA. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Dassoulas, J. A.; Dietrich, J.; Ferrara, V.; Friedrich, C.; Glazov, A.; Goebel, M.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Hiller, K. H.; Huettmann, A.; Belenguer, M. Jimenez; Johnert, S.; Katzy, J.; Kono, T.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Cavalcanti, T. Perez; Petschull, D.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildts, M. A.; Yatsenko, E.; Yildirim, E.; Zhu, H.] DESY, Hamburg, Germany. [Argyropoulos, S.; Bloch, I.; Borroni, S.; Dassoulas, J. A.; Dietrich, J.; Ferrara, V.; Friedrich, C.; Glazov, A.; Goebel, M.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Hiller, K. H.; Huettmann, A.; Belenguer, M. Jimenez; Johnert, S.; Katzy, J.; Kono, T.; Kuhl, T.; Lange, C.; Lisovyi, M.; Lobodzinska, E.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Cavalcanti, T. Perez; Petschull, D.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildts, M. A.; Yatsenko, E.; Yildirim, E.; Zhu, H.] DESY, Zeuthen, Germany. [Bunse, M.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Reisinger, I.; Wittig, T.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Czodrowski, P.; Friedrich, F.; Grohs, J. P.; Kobel, M.; Leonhardt, K.; Mader, W. F.; Morgenstern, M.; Prudent, X.; Rudolph, C.; Schnoor, U.; Seifert, F.; Steinbach, P.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B.; Finelli, K. D.; Ko, B. R.; Kotwal, A.; Liu, M.; Oh, S. H.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Buckley, A. G.; Clark, P. J.; Debenedetti, C.; Walls, F. M. Garay; Harrington, R. D.; Korn, A.; Kruse, M. K.; Martin, V. J.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Schaelicke, A.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.; Volpi, G.] INFN Lab Nazionali Frascati, Frascati, Italy. [Aad, G.; Ahles, F.; Amoroso, S.; Barber, T.; Bernhard, R.; Boehler, M.; Bruneliere, R.; Christov, A.; Consorti, V.; Fehling-Kaschek, M.; Flechl, M.; Giuliani, C.; Hartert, J.; Herten, G.; Jakobs, K.; Janus, M.; Jovicevic, J.; Kononov, A. I.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Lohwasser, K.; Ludwig, I.; Ludwig, J.; Madar, R.; Mahboubi, K.; Mohr, W.; Parzefall, U.; Rammensee, M.; Rave, T. C.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Siegert, F.; Stoerig, K.; Sundermann, J. E.; Temming, K. K.; Thoma, S.; Tsiskaridze, V.; Ungaro, F. C.; Venturi, M.; Vivarelli, I.; Von Radziewski, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Winkelmann, S.; Xie, S.; Zimmermann, S.] Univ Freiburg, Fak Mathemat & Phys, D-79106 Freiburg, Germany. [Abdelalim, A. A.; Alexandre, G.; Backes, M.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; Bucci, F.; Toro, R. Camacho; Clark, A.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Guescini, F.; Iacobucci, G.; La Rosa, A.; Latour, B. Martin Dit; Mermod, P.; Herrera, C. Mora; Nektarijevic, S.; Nikolics, K.; Asztorah, G. P.; Picazio, A.; Pohl, M.; Rosbach, K.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Beccherle, R.; Caso, C.; Darbo, G.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] INFN Sez Genova, Genoa, Italy. [Barberis, D.; Caso, C.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Khubua, J.; Mchedlidze, G.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Phys Inst 2, D-35390 Giessen, Germany. [Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Bussey, P.; Buttar, C. M.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Edwards, N. C.; Ferrag, S.; Ferrando, J.; De Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Kar, D.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Quilty, D.; Ravenscroft, T.; Robson, A.; Saxon, D. H.; Smith, K. M.; St Denis, R. D.; Steele, G.; Thompson, A. S.; Wraight, K.; Wright, M.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bierwagen, K.; Blumenschein, U.; Brandt, O.; Evangelakou, D.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Hensel, C.; Kawamura, G.; Keil, M.; Knue, A.; Kohn, F.; Krieger, N.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Meyer, J.; Morel, J.; Nackenhorst, O.; Pashapour, S.; Peters, R. F. Y.; Quadt, A.; Roe, A.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Schroeder, T. Vazquez; Weingarten, J.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocm, B.] Univ Grenoble 1, Lab Phys Subatom & Cosmol, Grenoble, France. [Albrand, S.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocm, B.] CNRS, IN2P3, Grenoble, France. [Albrand, S.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Sun, X.; Trocm, B.] Inst Natl Polytech Grenoble, F-38031 Grenoble, France. [Addy, T. N.; Harvey, A.; McFarlane, K. W.; Shin, T.; Vassilakopoulos, V. I.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Belloni, A.; Butler, B.; Catastini, P.; Conti, G.; Franklin, M.; Huth, J.; Jeanty, L.; Kagan, M.; Mateos, D. Lopez; Mercurio, K. M.; Mills, C.; Morii, M.; Skottowe, H. P.; Yen, A. L.; Della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Anders, G.; Andrei, V.; Davygora, Y.; Dietzsch, T. A.; Dunford, M.; Hanke, P.; Henke, M.; Hofmann, J. I.; Khomich, A.; Kluge, E. -E.; Laier, H.; Lang, V. S.; Lendermann, V.; Lepold, F.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Phys Inst, Heidelberg, Germany. [Kugel, A.; Schroer, N.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Evans, H.; Gagnon, P.; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Price, D.; Whittington, D.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jussel, P.; Kneringer, E.; Lukas, W.; Ritsch, E.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Cinca, D.; Gandrajula, R. P.; Halladjian, G.; Limper, M.; Mallik, U.; Mandrysch, R.; Morange, N.; Pylypchenko, Y.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Aleksandrov, I. N.; Bardin, D. Y.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Grigalashvili, N.; Huseynov, N.; Kazarinov, M. Y.; Kharchenko, D.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rumyantsev, L.; Rusakovich, N. A.; Sadykov, R.; Shiyakova, M.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.; Zimin, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Arai, Y.; Doi, Y.; Haruyama, T.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Makida, Y.; Mitsui, S.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] Natl Lab High Energy Phys, KEK, High Energy Accelerator Res Org, Tsukuba, Ibaraki 305, Japan. [Errede, S.; Hayakawa, T.; King, M.; Kishimoto, T.; Kitamura, T.; Kurashige, H.; Matsushita, T.; Ochi, A.; Suzuki, Y.; Takeda, H.; Tani, K.; Watanabe, I.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo, Japan. [Ishino, M.; Sasao, N.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.; Vos, M.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Loh, C. W.; Oda, S.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Verzini, M. J. Alconada; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Verzini, M. J. Alconada; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Allison, L. J.; Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Bianco, M.; Cataldi, G.; Chiodini, G.; Gorini, E.; Grancagnolo, F.; Orlando, N.; Perrino, R.; M., Primavera; Spagnolo, S.; Ventura, A.] INFN Sez Lecce, Lecce, Italy. [Bianco, M.; Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Greenshaw, T.; Gwilliam, C. B.; Hayward, H. S.; Jackson, J. N.; King, B. T.; Klein, M.; Kretzschmar, J.; Laycock, P.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Sellers, G.; Vossebeld, J. H.; Waller, P.; Wrona, B.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kashif, L.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kashif, L.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia. [Bona, M.; Carter, A. A.; Cerrito, L.; Eisenhandler, E.; Ellis, K.; Fletcher, G.; Goddard, J. R.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Rizvi, E.; Salamanna, G.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Baker, S.; Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Chislett, R. T.; Christidi, I. A.; Cooper, B. D.; Davison, A. R.; Dobson, E.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Lambourne, L.; Nash, M.; Nurse, E.; Ochoa, M. I.; Pilkington, A. D.; Prabhu, R.; Sherwood, P.; Simmons, B.; Taylor, C.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Bernius, C.; Dhullipudi, R.; Greenwood, Z. D.; Sawyer, L.; Sircar, A.; Subramaniam, R.; Tamsettam, M. C.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] Univ Paris 06, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Rangel-Smith, C.; Ridel, M.; Roos, L.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Jarlskog, G.; Lytken, E.; Meirose, B.; Mjoernmark, J. U.; Smirnova, O.; Wielers, M.] Lund Univ, Fys Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Labarga, L.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Arnaez, O.; Blum, W.; Buescher, V.; Caputo, R.; Eckweiler, S.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Goeringer, C.; Handel, C.; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Ji, W.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lungwitz, M.; Masetti, L.; Meyer, C.; Moreno, D.; Moritz, S.; Mueller, T.; Neusiedl, A.; Poettgen, R.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, D-55122 Mainz, Germany. [Almond, J.; Borri, M.; Brown, G.; Chavda, V.; Cox, B. E.; Da Via, C.; Forti, A.; Howarth, J.; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Marx, M.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Robinson, J. E. M.; Tomlinson, L.; Watts, S.; Woudstra, M. J.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Barbero, M.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Nagai, Y.; Odier, J.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Tothah, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Barbero, M.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Nagai, Y.; Odier, J.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Tothah, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Brau, B.; Colon, G.; Dallapiccola, C.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Sander, H. G.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Dufour, M-A.; Klemetti, M.; Mantifel, R.; Robertson, S. H.; Schram, M.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Davidson, N.; Diglio, S.; Hamano, K.; Jennens, D.; Kubota, T.; Limosani, A.; Hanninger, G. Nunes; Phan, A.; Shao, Q. T.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Volpi, M.; White, M. J.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Armbruster, A. J.; Chapman, J. W.; Cirilli, M.; Dai, T.; Diehl, E. B.; Dubbert, J.; Feng, H.; Ferretti, C.; Goldfarb, S.; Harper, D.; Levin, D.; Li, X.; Liu, L.; Mc Kee, S. P.; Neal, H. A.; Panikashvili, N.; Qian, J.; Scheirich, D.; Searcy, J.; Thun, R. P.; Walch, S.; Wilson, A.; Wooden, G.; Wu, Y.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Hauser, R.; Holzbauer, J. L.; Huston, J.; Koll, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schwienhorst, R.; Stelzer, H. J.; Tollefson, K.; True, P.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alessandria, F.; Alimonti, G.; Andreazza, A.; Besana, M. I.; Broggi, F.; Carminati, L.; Cavalli, D.; Citterio, M.; Coelli, S.; Consonni, S. M.; Costa, G.; Fanti, M.; Favareto, A.; Giugni, D.; Koletsou, I.; Lari, T.; Mandelli, L.; Mazzanti, M.; Meloni, F.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Rivoltella, G.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Volpini, G.] INFN Sez Milano, Milan, Italy. [Andreazza, A.; Besana, M. I.; Carminati, L.; Consonni, S. M.; Fanti, M.; Favareto, A.; Meloni, F.; Perini, L.; Pizio, C.; Ragusa, F.; Rivoltella, G.; Simoniello, R.; Turra, R.] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Satsounkevitch, I.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Asbah, N.; Azuelos, G.; Banerjee, P.; Bouchami, J.; Dallaire, F.; Davies, M.; Gauthier, L.; Giunta, M.; Leroy, C.; Martin, J. P.; Rezvani, R.; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.] Acad Sci, PN Lebedev Inst Phys, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys ITEP, Moscow, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.] Moscow Engn & Phys Inst MEPhI, Moscow, Russia. [Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnovaak, L. N.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Biebel, O.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; de Graat, J.; Duckeck, G.; Ebke, J.; Elmsheuser, J.; Engl, A.; Galea, C.; Heller, C.; Hertenberger, R.; Legger, F.; Lorenz, J.; Mann, A.; Meineck, C.; Oakes, L. B.; Rauscher, F.; Reznicek, P.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Schieck, J.; Staude, A.; Vladoiu, D.; Will, J. Z.; Wittkowski, J.; Zibell, A.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bittner, B.; Bronner, J.; Capriotti, D.; Compostella, G.; Cortiana, G.; Flowerdew, M. J.; Giovannini, P.; Goblirsch-Kolb, M.; Ince, T.; Jantsch, A.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kotov, S.; Kroha, H.; Macchiolo, A.; Manfredini, A.; Menke, S.; Moser, H. G.; Nagel, M.; Nisius, R.; Oberlack, H.; Pahl, C.; Pospelov, G. E.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Stern, S.; Stonjek, S.; Vanadia, M.; Von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Shimizu, S.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Shimizu, S.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Della Volpe, D.; Di Donato, C.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Patricelli, S.; Sanchez, A.; Sekhniaidze, G.] INFN Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Chiefari, G.; Della Volpe, D.; Di Donato, C.; Giordano, R.; Merola, L.; Patricelli, S.; Sanchez, A.] Univ Naples Federico II, Dipartimento Sci Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Chelstowska, M. A.; Dao, V.; De Groot, N.; Filthaut, F.; Klok, P. F.; Koetsveld, F.; Koenig, A. C.; Raas, M.; Salvucci, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Pani, P.; Ruckstuhl, N.; Ta, D.; Tsiakiris, M.; Valencic, N.; Van der Deijl, P. C.; Van der Geer, R.; Van der Graaf, H.; Van der Leeuw, R.; Van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Pani, P.; Ruckstuhl, N.; Ta, D.; Tsiakiris, M.; Valencic, N.; Van der Deijl, P. C.; Van der Geer, R.; Van der Graaf, H.; Van der Leeuw, R.; Van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.] Univ Amsterdam, Amsterdam, Netherlands. [Calkins, R.; Chakraborty, D.; Cole, S.; De Lima, J. G. Rocha; Suhr, C.; Yurkewicz, A.; Zutshi, V.] Univ Illinois, Dept Phys, De Kalb, IL USA. [Anisenkov, A. V.; Beloborodova, O. L.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Skovpen, K. Yu.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Budick, B.; Casadei, D.; Cranmer, K.; Haas, A.; Van Huysduynen, L. Hooft; Kaplan, B.; Konoplich, R.; Krasznahorkay, A.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.; Prokofiev, K.] NYU, Dept Phys, New York, NY 10003 USA. [Fisher, M. J.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Strang, M.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama, Japan. [Abbott, B.; Gutierrez, P.; Jana, D. K.; Marzin, A.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Snow, J.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Khanov, A.; Meera-Lebbai, R.; Rizatdinova, F.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Hamal, P.; Hrabovsky, M.; Nozka, L.] Palack Univ, RCPTM, Olomouc, Czech Republic. [Brau, J. E.; Brost, E.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Reinsch, A.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Auge, E.; Binet, S.; Bourdarios, C.; De La Taille, C.; De Regie, J. B. De Vivie; Duot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Henrot-Versille, S.; Herbert, G. H.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Niedercorn, F.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Teinturier, M.; Tran, H. L.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Auge, E.; Binet, S.; Bourdarios, C.; De La Taille, C.; De Regie, J. B. De Vivie; Duot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Henrot-Versille, S.; Herbert, G. H.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Niedercorn, F.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Teinturier, M.; Tran, H. L.; Zerwas, D.; Zhang, Z.] CNRS, IN2P3, Orsay, France. [Hanagaki, K.; Hirose, M.; Lee, J. S. H.; Meguro, T.; Nomachi, M.; Okamura, W.; Sugaya, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Buran, T.; Cameron, D.; Gjelsten, B. K.; Gramstad, E.; Lund, E.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Read, A. L.; Rohne, O.; Smestad, L.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Apolle, R.; Barr, A. J.; Boddy, C. R.; Buchanan, J.; Buckingham, R. M.; Cooper-Sarkar, A. M.; Dafinca, A.; Davies, E.; Gallas, E. J.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; King, R. S. B.; Kogan, L. A.; Larner, A.; Lewis, A.; Liang, Z.; Livermore, S. S. A.; Mattravers, C.; Nickerson, R. B.; Pinder, A.; Robichaud-Veronneau, A.; Ryder, N. C.; Sawyer, C.; Short, D.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Whitehead, S. R.; Young, C. J. S.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Colombo, T.; Conta, C.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] INFN Sez Pavia, Pavia, Italy. [Colombo, T.; Conta, C.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Degenhardt, J.; Hines, E.; Jackson, B.; Keener, P. T.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Newcomer, F. M.; Olivito, D.; Ospanov, R.; Saxon, J.; Schaefer, D.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Bertolucci, F.; Cascella, M.; Cavasinni, V.; Del Prete, T.; Dotti, A.; Giannetti, P.; Roda, C.; Sarri, F.; White, S.; Zinonos, Z.] INFN Sez Pisa, Pisa, Italy. [Bertolucci, F.; Cascella, M.; Cavasinni, V.; Del Prete, T.; Dotti, A.; Giannetti, P.; Roda, C.; Sarri, F.; White, S.; Zinonos, Z.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Escobar, C.; Kittelmann, T.; Mueller, J.; Prieur, D.; Sapp, K.; Savinov, V.; Yoosoofmiya, R.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [dos Santos, S. P. Amor; Amorim, A.; Anjos, N.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; De Sousa, M. J. Da Cunha Sargedas; Wemans, A. Do Valle; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Jorge, P. M.; Lopes, L.; Miguens, J. Machado; Maio, A.; Maneira, J.; Marques, C. N.; Oliveira, M.; Onofre, A.; Palma, A.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Veloso, F.; Wolters, H.] Lab Instrumentacao Fis Expt Particulas LIP, Lisbon, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. [Bohm, J.; Chudoba, J.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Myska, M.; Nemecek, S.; Ruzicka, P.; Schovancova, J.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Tic, T.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Gallus, P.; Gunther, J.; Jakubek, J.; Kohout, Z.; Kral, V.; Pospisil, S.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solar, M.; Solc, J.; Sopko, V.; Sopko, B.; Stekl, I.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, Prague, Czech Republic. [Balek, P.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Torregrosa, E. Fullana; Kodys, P.; Leitner, R.; Novakova, J.; Pleskot, V.; Rybar, M.; Spoustaal, M.; Sykora, T.; Tas, P.; Valkar, S.; Vorobel, V.; Wilhelm, I.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Ammosov, V. V.; Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Ivashin, V.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.; Zmouchko, V. V.] State Res Ctr Inst High Energy Phys, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Gillman, A. R.; Haywood, S. J.; Kirk, J.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Tyndel, M.; Wickens, F. J.] Rutherford Appleton Lab, Particle Phys Dept, Didcot, Oxon, England. [Benslama, K.] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Shiga, Japan. [Anulli, F.; Artoni, G.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Pedis, D.; De Salvo, A.; De Zorzi, G.; Dionisi, C.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; Losterzo, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Rossi, E.; Tehrani, F. Safai; Sidoti, A.; Camillocci, E. Solfaroli; Vari, R.; Veneziano, S.; Zanello, L.] INFN Sez Roma I, Rome, Italy. [Artoni, G.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Zorzi, G.; Dionisi, C.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; Losterzo, F.; Luci, C.; Rossi, E.; Camillocci, E. Solfaroli; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Di Simone, A.; Liberti, B.; Marchese, F.; Mazzaferro, L.; Salamon, A.; Santonico, R.] INFN Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Cattani, G.; Di Ciaccio, A.; Di Simone, A.; Marchese, F.; Mazzaferro, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Rome, Italy. [Damiani, D. S.; Grillo, A. A.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Mitrevski, J.; Nielsen, J.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Beckingham, M.; Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Hsu, S. -C.; Keller, J. S.; Lubatti, H. J.; Rompotis, N.; Rothberg, J.; Verducci, M.; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Mcfayden, J. A.; Miyagawa, P. S.; Owen, S.; Paganis, E.; Suruliz, K.; Tovey, D. R.; Tua, A.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Ibragimov, I.; Ikematsu, K.; Rammes, M.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Dawe, E.; Godfrey, J.; Kvita, J.; O'Neil, D. C.; Petteni, M.; Stelzer, B.; Tanasijczuk, A. J.; Trottier-McDonald, M.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Mayes, J. Backus; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Hansson, P.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nelson, T. K.; Piacquadio, G.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Strauss, E.; Su, D.; Swiatlowski, M.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Ahmad, A.; Arfaoui, S.; DeWilde, B.; Engelmann, R.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Puldon, D.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Bartsch, V.; De Santo, A.; Martin-Haugh, S.; Potter, C. J.; Rose, A.; Salvatore, F.; Castillo, I. Santoyo; Sutton, M. R.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Bangert, A.; Black, C. W.; Cuthbert, C.; Jeng, G. -Y.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Waugh, A. T.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Chu, M. L.; Hou, S.; Jamin, D. O.; Lee, S. C.; Lin, S. C.; Liu, D.; Mazini, R.; Ren, Z. L.; Soh, D. A.; Teng, P. K.; Wang, J.; Wang, S. M.; Weng, Z.; Zhang, L.; Zhou, Y.] Acad Sinica, Inst Phys, Taipei 115, Taiwan. [Di Mattia, A.; Kajomovitz, E.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; Vallecorsa, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Bella, G.; Benary, O.; Benhammou, Y.; Etzion, E.; Gershon, A.; Gueta, O.; Guttman, N.; Munwes, Y.; Oren, Y.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkialas, I.; Iliadis, D.; Kordas, K.; Kouskoura, V.; Nomidis, I.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamaguchi, Y.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yamazaki, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Dohmae, T.; Kanaya, N.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, T.; Okuyama, T.; Sakamoto, H.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Basye, A.] Kings Coll London, Dept Phys, London, England. [Amorim, A.; Gomes, A.; Maio, A.; Pina, J.] Univ Lisbon, Fac Ciencias, P-1699 Lisbon, Portugal. [Amorim, A.; Gomes, A.; Maio, A.; Pina, J.] Univ Lisbon, CFNUL, P-1699 Lisbon, Portugal. [Apolle, R.; Davies, E.; Mattravers, C.; Nash, M.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot, Oxon, England. [Azuelos, G.; Gingrich, D. M.; Oakham, F. G.; Savard, P.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Bawa, H. S.; Gao, Y. S.; Lowe, A. J.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beloborodova, O. L.; Maximov, D. A.; Talyshev, A. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk, Russia. [Carvalho, J.; Fiolhais, M. C. N.; Oliveira, M.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Demirkoz, B.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Dhullipudi, R.; Greenwood, Z. D.; Sawyer, L.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Wemans, A. Do Valle] Univ Nova Lisboa, Dep Fis, Fac Ciencias & Tecnol, Caparica, Portugal. [Wemans, A. Do Valle] Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, Caparica, Portugal. [Ge, P.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Gkialas, I.; Papageorgiou, K.] Univ Aegean, Dept Financial & Management Engn, Chios, Greece. [Grinstein, S.; Rozas, A. Juste; Martinez, M.] Inst Catalana Recerca & Estudis Avancats, ICREA, Barcelona, Spain. [Kono, T.; Wildts, M. A.] Azerbaijan Acad Sci, Inst Phys, Baku 370143, Azerbaijan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Li, B.; Li, S.] Acad Sinica, Inst Phys, Taipei, Taiwan. RP Aad, G (reprint author), Univ Freiburg, Fak Mathemat & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. RI Fassi, Farida/F-3571-2016; la rotonda, laura/B-4028-2016; Karyukhin, Andrey/J-3904-2014; Capua, Marcella/A-8549-2015; Tartarelli, Giuseppe Francesco/A-5629-2016; KHODINOV, ALEKSANDR/D-6269-2015; Goncalo, Ricardo/M-3153-2016; Gauzzi, Paolo/D-2615-2009; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Yang, Haijun/O-1055-2015; Monzani, Simone/D-6328-2017; Grancagnolo, Francesco/K-2857-2015; Korol, Aleksandr/A-6244-2014; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Vykydal, Zdenek/H-6426-2016; Olshevskiy, Alexander/I-1580-2016; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Mora Herrera, Maria Clemencia/L-3893-2016; Maneira, Jose/D-8486-2011; Prokoshin, Fedor/E-2795-2012; Gavrilenko, Igor/M-8260-2015; Akimov, Andrey/N-1769-2015; Tikhomirov, Vladimir/M-6194-2015; Chekulaev, Sergey/O-1145-2015; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; Andreazza, Attilio/E-5642-2011; Mashinistov, Ruslan/M-8356-2015; Buttar, Craig/D-3706-2011; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Cabrera Urban, Susana/H-1376-2015; Mir, Lluisa-Maria/G-7212-2015; Della Pietra, Massimo/J-5008-2012; Cavalli-Sforza, Matteo/H-7102-2015; Petrucci, Fabrizio/G-8348-2012; Negrini, Matteo/C-8906-2014; Ferrer, Antonio/H-2942-2015; Hansen, John/B-9058-2015; Grancagnolo, Sergio/J-3957-2015; spagnolo, stefania/A-6359-2012; Ciubancan, Liviu Mihai/L-2412-2015; Shmeleva, Alevtina/M-6199-2015; Camarri, Paolo/M-7979-2015; Gabrielli, Alessandro/H-4931-2012; Marti-Garcia, Salvador/F-3085-2011; Shabalina, Elizaveta/M-2227-2013; Ferrando, James/A-9192-2012; Snesarev, Andrey/H-5090-2013; Warburton, Andreas/N-8028-2013; Sukharev, Andrey/A-6470-2014; Doyle, Anthony/C-5889-2009; Moraes, Arthur/F-6478-2010; Boyko, Igor/J-3659-2013; Brooks, William/C-8636-2013; Wolters, Helmut/M-4154-2013; Castro, Nuno/D-5260-2011; Grinstein, Sebastian/N-3988-2014; Wemans, Andre/A-6738-2012; Demirkoz, Bilge/C-8179-2014; Gutierrez, Phillip/C-1161-2011; Ventura, Andrea/A-9544-2015; Livan, Michele/D-7531-2012; De, Kaushik/N-1953-2013; Mitsou, Vasiliki/D-1967-2009; White, Ryan/E-2979-2015; Joergensen, Morten/E-6847-2015; Riu, Imma/L-7385-2014; Jakoubek, Tomas/G-8644-2014; Staroba, Pavel/G-8850-2014; Kupco, Alexander/G-9713-2014; de Groot, Nicolo/A-2675-2009; Hejbal, Jiri/H-1358-2014; Marcisovsky, Michal/H-1533-2014; Mikestikova, Marcela/H-1996-2014; Lysak, Roman/H-2995-2014; Tomasek, Lukas/G-6370-2014; Svatos, Michal/G-8437-2014; Chudoba, Jiri/G-7737-2014; Peleganchuk, Sergey/J-6722-2014; Bosman, Martine/J-9917-2014; Solfaroli Camillocci, Elena/J-1596-2012; Lee, Jason/B-9701-2014; Robson, Aidan/G-1087-2011; Kuday, Sinan/C-8528-2014; Smirnova, Oxana/A-4401-2013; Zimmermann, Claus/E-9598-2014; Fabbri, Laura/H-3442-2012; Villa, Mauro/C-9883-2009; Carvalho, Joao/M-4060-2013; Nozka, Libor/G-5550-2014; Nemecek, Stanislav/G-5931-2014; Kepka, Oldrich/G-6375-2014; Lokajicek, Milos/G-7800-2014 OI Gomes, Agostinho/0000-0002-5940-9893; Fassi, Farida/0000-0002-6423-7213; la rotonda, laura/0000-0002-6780-5829; Osculati, Bianca Maria/0000-0002-7246-060X; Amorim, Antonio/0000-0003-0638-2321; Santos, Helena/0000-0003-1710-9291; Coccaro, Andrea/0000-0003-2368-4559; Fiolhais, Miguel/0000-0001-9035-0335; Karyukhin, Andrey/0000-0001-9087-4315; Anjos, Nuno/0000-0002-0018-0633; Smestad, Lillian/0000-0002-0244-8736; Giordani, Mario/0000-0002-0792-6039; Abdelalim, Ahmed Ali/0000-0002-2056-7894; Capua, Marcella/0000-0002-2443-6525; Di Micco, Biagio/0000-0002-4067-1592; Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; Doria, Alessandra/0000-0002-5381-2649; Veloso, Filipe/0000-0002-5956-4244; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Goncalo, Ricardo/0000-0002-3826-3442; Gauzzi, Paolo/0000-0003-4841-5822; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Monzani, Simone/0000-0002-0479-2207; Grancagnolo, Francesco/0000-0002-9367-3380; Korol, Aleksandr/0000-0001-8448-218X; Maio, Amelia/0000-0001-9099-0009; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Vykydal, Zdenek/0000-0003-2329-0672; Olshevskiy, Alexander/0000-0002-8902-1793; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; Tikhomirov, Vladimir/0000-0002-9634-0581; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; Andreazza, Attilio/0000-0001-5161-5759; Mashinistov, Ruslan/0000-0001-7925-4676; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Mir, Lluisa-Maria/0000-0002-4276-715X; Della Pietra, Massimo/0000-0003-4446-3368; Petrucci, Fabrizio/0000-0002-5278-2206; Negrini, Matteo/0000-0003-0101-6963; Ferrer, Antonio/0000-0003-0532-711X; Hansen, John/0000-0002-8422-5543; Grancagnolo, Sergio/0000-0001-8490-8304; spagnolo, stefania/0000-0001-7482-6348; Ciubancan, Liviu Mihai/0000-0003-1837-2841; Camarri, Paolo/0000-0002-5732-5645; Gabrielli, Alessandro/0000-0001-5346-7841; Ferrando, James/0000-0002-1007-7816; Warburton, Andreas/0000-0002-2298-7315; Doyle, Anthony/0000-0001-6322-6195; Moraes, Arthur/0000-0002-5157-5686; Boyko, Igor/0000-0002-3355-4662; Brooks, William/0000-0001-6161-3570; Wolters, Helmut/0000-0002-9588-1773; Castro, Nuno/0000-0001-8491-4376; Grinstein, Sebastian/0000-0002-6460-8694; Wemans, Andre/0000-0002-9669-9500; Ventura, Andrea/0000-0002-3368-3413; Livan, Michele/0000-0002-5877-0062; De, Kaushik/0000-0002-5647-4489; Mitsou, Vasiliki/0000-0002-1533-8886; White, Ryan/0000-0003-3589-5900; Joergensen, Morten/0000-0002-6790-9361; Riu, Imma/0000-0002-3742-4582; Mikestikova, Marcela/0000-0003-1277-2596; Tomasek, Lukas/0000-0002-5224-1936; Svatos, Michal/0000-0002-7199-3383; Peleganchuk, Sergey/0000-0003-0907-7592; Bosman, Martine/0000-0002-7290-643X; Solfaroli Camillocci, Elena/0000-0002-5347-7764; Lee, Jason/0000-0002-2153-1519; Kuday, Sinan/0000-0002-0116-5494; Smirnova, Oxana/0000-0003-2517-531X; Fabbri, Laura/0000-0002-4002-8353; Villa, Mauro/0000-0002-9181-8048; Carvalho, Joao/0000-0002-3015-7821; FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union; ERC, European Union; NSRF, European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; ISF, Israel; MINERVA, Israel; GIF, Israel; DIP, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; GRICES, Portugal; FCT, Portugal; MERYS (MECTS), Romania; MES of Russia, Russian Federation; ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Cantons of Bern, Switzerland; Cantons of Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; ISF, MINERVA, GIF, DIP and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW, Poland; GRICES and FCT, Portugal; MERYS (MECTS), Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. NR 58 TC 1 Z9 1 U1 6 U2 135 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD OCT 8 PY 2013 IS 10 AR UNSP 042 DI 10.1007/JHEP10(2013)042 PG 38 WC Physics, Particles & Fields SC Physics GA 232LW UT WOS:000325496300001 ER PT J AU Bevc, S Junghans, C Kremer, K Praprotnik, M AF Bevc, Stas Junghans, Christoph Kremer, Kurt Praprotnik, Matej TI Adaptive resolution simulation of salt solutions SO NEW JOURNAL OF PHYSICS LA English DT Article ID MOLECULAR-DYNAMICS INTEGRATION; MONTE-CARLO-SIMULATION; COARSE-GRAINED MODEL; MULTISCALE SIMULATION; BIOMOLECULAR SIMULATIONS; VIBRATIONAL THEORY; FORCE-FIELDS; SOFT MATTER; FLUID-FLOWS; WATER AB We present an adaptive resolution simulation of aqueous salt (NaCl) solutions at ambient conditions using the adaptive resolution scheme. Our multiscale approach concurrently couples the atomistic and coarse-grained models of the aqueous NaCl, where water molecules and ions change their resolution while moving from one resolution domain to the other. We employ standard extended simple point charge (SPC/E) and simple point charge (SPC) water models in combination with AMBER and GROMOS force fields for ion interactions in the atomistic domain. Electrostatics in our model are described by the generalized reaction field method. The effective interactions for water-water and water-ion interactions in the coarse-grained model are derived using structure-based coarse-graining approach while the Coulomb interactions between ions are appropriately screened. To ensure an even distribution of water molecules and ions across the simulation box we employ thermodynamic forces. We demonstrate that the equilibrium structural, e.g. radial distribution functions and density distributions of all the species, and dynamical properties are correctly reproduced by our adaptive resolution method. Our multiscale approach, which is general and can be used for any classical non-polarizable force-field and/or types of ions, will significantly speed up biomolecular simulation involving aqueous salt. C1 [Bevc, Stas; Praprotnik, Matej] Natl Inst Chem, SI-1001 Ljubljana, Slovenia. [Junghans, Christoph] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Kremer, Kurt] Max Planck Inst Polymer Res, D-55128 Mainz, Germany. RP Kremer, K (reprint author), Max Planck Inst Polymer Res, Ackermannweg 10, D-55128 Mainz, Germany. EM kremer@mpip-mainz.mpg.de; praprot@cmm.ki.si RI Junghans, Christoph/G-4238-2010; Kremer, Kurt/G-5652-2011; MPIP, Theory/I-9884-2014 OI Junghans, Christoph/0000-0003-0925-1458; FU National Science Foundation [NSF PHY11-25915]; Slovenian Research Agency [J1-2281, J1-4134, P1-0002]; LANL FX We thank Luigi Delle Site for useful discussions and acknowledge hospitality at KITP. This research was supported in part by the National Science Foundation under grant number NSF PHY11-25915. SB and MP acknowledge financial support through the grant numbers J1-2281, J1-4134 and P1-0002 from the Slovenian Research Agency. CJ thanks LANL for a Director's fellowship. NR 73 TC 14 Z9 14 U1 1 U2 29 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1367-2630 J9 NEW J PHYS JI New J. Phys. PD OCT 8 PY 2013 VL 15 AR 105007 DI 10.1088/1367-2630/15/10/105007 PG 12 WC Physics, Multidisciplinary SC Physics GA 230FL UT WOS:000325322000005 ER PT J AU Kondo, T Palczewski, AD Hamaya, Y Takeuchi, T Wen, JS Xu, ZJ Gu, G Kaminski, A AF Kondo, Takeshi Palczewski, Ari D. Hamaya, Yoichiro Takeuchi, Tsunehiro Wen, J. S. Xu, Z. J. Gu, Genda Kaminski, Adam TI Formation of Gapless Fermi Arcs and Fingerprints of Order in the Pseudogap State of Cuprate Superconductors SO PHYSICAL REVIEW LETTERS LA English DT Article ID HIGH-T-C; UNDERDOPED BI2SR2CACU2O8+DELTA; DYNAMICS; DENSITY; ORIGIN AB We use angle-resolved photoemission spectroscopy and a new quantitative approach based on the partial density of states to study properties of seemingly disconnected portions of the Fermi surface (FS) that are present in the pseudogap state of cuprates called Fermi arcs. We find that the normal state FS collapses very abruptly into Fermi arcs at the pseudogap temperature (T*). Surprisingly, the length of the Fermi arcs remains constant over an extended temperature range between T* and T-pair, consistent with the presence of an ordered state below T*. These arcs collapse again at the temperature below which pair formation occurs (T-pair) either to a point or a very short arc, whose length is limited by our experimental resolution. The tips of the arcs span between points defining a set of wave vectors in momentum space, which are the fingerprints of the ordered state that causes the pseudogap. C1 [Kondo, Takeshi; Palczewski, Ari D.; Kaminski, Adam] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. [Kondo, Takeshi; Palczewski, Ari D.; Kaminski, Adam] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Hamaya, Yoichiro; Takeuchi, Tsunehiro] Nagoya Univ, Dept Crystalline Mat Sci, Nagoya, Aichi 4648603, Japan. [Takeuchi, Tsunehiro] Nagoya Univ, EcoTopia Sci Inst, Nagoya, Aichi 4648603, Japan. [Wen, J. S.; Xu, Z. J.; Gu, Genda] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RP Kondo, T (reprint author), Univ Tokyo, Inst Solid State Phys, Kashiwa, Chiba 2778581, Japan. RI Wen, Jinsheng/F-4209-2010; xu, zhijun/A-3264-2013; Kondo, Takeshi/H-2680-2016 OI Wen, Jinsheng/0000-0001-5864-1466; xu, zhijun/0000-0001-7486-2015; FU Basic Energy Sciences, U.S. DOE; JSPS (KAKENHI) [24740218]; U.S. DOE by Iowa State University [DE-AC02-07CH11358]; U.S. DOE [DE-AC02-98CH10886]; Center for Emergent Superconductivity, an Energy Frontier Research Center; U.S. DOE, Office of Science FX We thank Mike Norman, Jorg Schmalian, and Andrey V. Chubukov for useful discussions. This work was supported by Basic Energy Sciences, U.S. DOE. T. K. is supported by JSPS (KAKENHI Contract No. 24740218). The Ames Laboratory is operated for the U.S. DOE by Iowa State University under Contract No. DE-AC02-07CH11358. Work at Brookhaven is supported by the U.S. DOE under Contract No. DE-AC02-98CH10886. J. S. W. and Z. J. X. are supported by the Center for Emergent Superconductivity, an Energy Frontier Research Center funded by the U.S. DOE, Office of Science. NR 34 TC 19 Z9 19 U1 3 U2 39 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 8 PY 2013 VL 111 IS 15 AR 157003 DI 10.1103/PhysRevLett.111.157003 PG 5 WC Physics, Multidisciplinary SC Physics GA 230VX UT WOS:000325372500009 PM 24160620 ER PT J AU Lee, CC Chen, XQM Gan, Y Yeh, CL Hsueh, HC Abbamonte, P Ku, W AF Lee, Chi-Cheng Chen, Xiaoqian M. Gan, Yu Yeh, Chen-Lin Hsueh, H. C. Abbamonte, Peter Ku, Wei TI First-Principles Method of Propagation of Tightly Bound Excitons: Verifying the Exciton Band Structure of LiF with Inelastic x-Ray Scattering SO PHYSICAL REVIEW LETTERS LA English DT Article ID ELECTRON-HOLE EXCITATIONS; INSULATORS; ABSORPTION; SPECTRA AB We propose a simple first-principles method to describe the propagation of tightly bound excitons. By viewing the exciton as a composite object (an effective Frenkel exciton in Wannier orbitals), we define an exciton kinetic kernel to encapsulate the exciton propagation and decay for all binding energies. Applied to prototypical LiF, our approach produces three exciton bands, which we verified quantitatively via inelastic x-ray scattering. The proposed real-space picture is computationally inexpensive and thus enables study of the full exciton dynamics, even in the presence of surfaces and impurity scattering. It also provides an intuitive understanding to facilitate practical exciton engineering in semiconductors, strongly correlated oxides, and their nanostructures. C1 [Lee, Chi-Cheng; Yeh, Chen-Lin; Ku, Wei] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Lee, Chi-Cheng] Acad Sinica, Inst Phys, Taipei 11529, Taiwan. [Chen, Xiaoqian M.; Gan, Yu; Abbamonte, Peter] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Chen, Xiaoqian M.; Gan, Yu; Abbamonte, Peter] Univ Illinois, Frederick Seitz Mat Res Lab, Urbana, IL 61801 USA. [Gan, Yu; Abbamonte, Peter] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Yeh, Chen-Lin; Hsueh, H. C.] Tamkang Univ, Dept Phys, Tamsui 25137, Taipei, Taiwan. RP Lee, CC (reprint author), Japan Adv Inst Sci & Technol JAIST, Sch Mat Sci, 1-1 Asahidai, Nomi, Ishikawa 9231292, Japan. EM abbamonte@mrl.illinois.edu; weiku@bnl.gov RI Lee, Chi-Cheng/F-5057-2015 OI Lee, Chi-Cheng/0000-0002-3895-9802 FU U.S. Department of Energy (DOE), Office of Basic Energy Science [DE-AC02-98CH10886]; DOE CMSN; DOE [DE-FG02-06ER46285, DE-AC02-O6CH11357]; National Science Council (NSC) [NSC 101-2112-M-032-001-MY3]; NCTS of Taiwan FX C.-C. L. is grateful for useful discussions with T.-K. Lee. Theoretical work is supported by the U.S. Department of Energy (DOE), Office of Basic Energy Science, under Contract No. DE-AC02-98CH10886 and DOE CMSN. IXS measurements are supported by DOE Grant No. DE-FG02-06ER46285. C.-C. L., C.-L. Y., and H. C. H. acknowledge support by the National Science Council (NSC under Contract No. NSC 101-2112-M-032-001-MY3) and NCTS of Taiwan. Use of the Advanced Photon Source is supported by DOE Contract No. DE-AC02-O6CH11357. Use of the National Center for High-Performance Computing of Taiwan is acknowledged. NR 27 TC 4 Z9 4 U1 3 U2 23 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 8 PY 2013 VL 111 IS 15 AR 157401 DI 10.1103/PhysRevLett.111.157401 PG 5 WC Physics, Multidisciplinary SC Physics GA 230VX UT WOS:000325372500011 PM 24160627 ER PT J AU Lin, YY Wen, JG Hu, LH Kennedy, RM Stair, PC Poeppelmeier, KR Marks, LD AF Lin, Yuyuan Wen, Jianguo Hu, Linhua Kennedy, Robert M. Stair, Peter C. Poeppelmeier, Kenneth R. Marks, Laurence D. TI Synthesis-Dependent Atomic Surface Structures of Oxide Nanoparticles SO PHYSICAL REVIEW LETTERS LA English DT Article ID SCANNING-TUNNELING-MICROSCOPY; SRTIO3(001) SURFACE; HYDROTHERMAL SYNTHESIS; HIGH-RESOLUTION; RECONSTRUCTIONS; MICROWAVE; NANOCUBOIDS; SCATTERING; ELECTRONS; TITANATE AB Using SrTiO3 nanocuboids as a model system, we show with aberration-corrected high resolution electron microscopy at sub-angstrom resolution that surface relaxations or reconstructions are present on the nanocuboids, depending on the synthetic process. Oleic acid synthesis, acetic acid synthesis, and microwave-assisted acetic acid synthesis result in a SrO termination, TiO2-rich reconstruction, and mixed termination, respectively. The experimental atomic positions are in better agreement with density functional theory calculations using an exact-exchange corrected PBEsol functional than the Perdew-Burke-Ernzerhof (PBE) functional. C1 [Lin, Yuyuan; Marks, Laurence D.] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. [Wen, Jianguo] Argonne Natl Lab, Electron Microscopy Ctr, Argonne, IL 60439 USA. [Hu, Linhua; Kennedy, Robert M.; Stair, Peter C.; Poeppelmeier, Kenneth R.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Stair, Peter C.; Poeppelmeier, Kenneth R.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Lin, YY (reprint author), Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. EM YuyuanLin2014@u.northwestern.edu; l-marks@northwestern.edu RI Marks, Laurence/B-7527-2009 FU Northwestern University Institute for Catalysis in Energy Processes (ICEP) [DOE DE-FG02-03-ER15457]; U.S. Department of Energy Office of Science Laboratory [DE-AC02-06CH11357]; Institute for Atom-Efficient Chemical Transformations (IACT), an Energy Frontier Research Center; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences FX We acknowledge funding from Northwestern University Institute for Catalysis in Energy Processes (ICEP) on Grant No. DOE DE-FG02-03-ER15457 (Y.L., L. H., P. C. S., K. R. P., and L. D. M.). The electron microscopy was performed at the Electron Microscopy Center for Materials Research at Argonne National Laboratory, a U.S. Department of Energy Office of Science Laboratory operated under Contract No. DE-AC02-06CH11357 by UChicago Argonne, LLC. R.K.'s work is based upon work supported as part of the Institute for Atom-Efficient Chemical Transformations (IACT), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. NR 45 TC 16 Z9 16 U1 2 U2 77 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 8 PY 2013 VL 111 IS 15 AR 156101 DI 10.1103/PhysRevLett.111.156101 PG 5 WC Physics, Multidisciplinary SC Physics GA 230VX UT WOS:000325372500006 PM 24160614 ER PT J AU Polei, S Snijders, PC Erwin, SC Himpsel, FJ Meiwes-Broer, KH Barke, I AF Polei, S. Snijders, P. C. Erwin, S. C. Himpsel, F. J. Meiwes-Broer, K-H. Barke, I. TI Structural Transition in Atomic Chains Driven by Transient Doping SO PHYSICAL REVIEW LETTERS LA English DT Article ID SCANNING-TUNNELING-MICROSCOPY; MOLECULAR-DYNAMICS; SURFACE; MANIPULATION; PHASE AB A reversible structural transition is observed on Si(553)-Au by scanning tunneling microscopy, triggered by electrons injected from the tip into the surface. The periodicity of atomic chains near the step edges changes from the 1 x 3 ground state to a 1 x 2 excited state with increasing tunneling current. The threshold current for this transition is reduced at lower temperatures. In conjunction with first-principles density-functional calculations it is shown that the 1 x 2 phase is created by temporary doping of the atom chains. Random telegraph fluctuations between two levels of the tunneling current provide direct access to the dynamics of the phase transition, revealing lifetimes in the millisecond range. C1 [Polei, S.; Meiwes-Broer, K-H.; Barke, I.] Univ Rostock, Dept Phys, D-18051 Rostock, Germany. [Snijders, P. C.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Snijders, P. C.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Erwin, S. C.] Naval Res Lab, Ctr Computat Mat Sci, Washington, DC 20375 USA. [Himpsel, F. J.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. RP Polei, S (reprint author), Univ Rostock, Dept Phys, D-18051 Rostock, Germany. EM ingo.barke@uni-rostock.de OI Meiwes-Broer, Karl-Heinz/0000-0002-8516-0470 FU federal state Mecklenburg-Vorpommern within the project Nano4Hydrogen; U.S. DOE Office of Basic Energy Sciences, Materials Sciences and Engineering Division, through the Oak Ridge National Laboratory; Office of Naval Research through the Naval Research Laboratory's Basic Research Program FX Funding by the federal state Mecklenburg-Vorpommern within the project Nano4Hydrogen is gratefully acknowledged (S. P., I. B., K. H. M.-B.). P. C. S. acknowledges support by the U.S. DOE Office of Basic Energy Sciences, Materials Sciences and Engineering Division, through the Oak Ridge National Laboratory. This work was supported by the Office of Naval Research through the Naval Research Laboratory's Basic Research Program (SCE). Computations were performed at the DOD Major Shared Resource Centers at AFRL and ERDC. I. B. acknowledges fruitful discussions with V. v. Oeynhausen and J. Tiggesbaumker. NR 47 TC 7 Z9 7 U1 2 U2 41 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 8 PY 2013 VL 111 IS 15 AR 156801 DI 10.1103/PhysRevLett.111.156801 PG 5 WC Physics, Multidisciplinary SC Physics GA 230VX UT WOS:000325372500008 PM 24160617 ER PT J AU Watanabe, H Lorusso, G Nishimura, S Xu, ZY Sumikama, T Soderstrom, PA Doornenbal, P Browne, F Gey, G Jung, HS Taprogge, J Vajta, Z Wu, J Yagi, A Baba, H Benzoni, G Chae, KY Crespi, FCL Fukuda, N Gernhauser, R Inabe, N Isobe, T Jungclaus, A Kameda, D Kim, GD Kim, YK Kojouharov, I Kondev, FG Kubo, T Kurz, N Kwon, YK Lane, GJ Li, Z Moon, CB Montaner-Piza, A Moschner, K Naqvi, F Niikura, M Nishibata, H Nishimura, D Odahara, A Orlandi, R Patel, Z Podolyak, Z Sakurai, H Schaffner, H Simpson, GS Steiger, K Suzuki, H Takeda, H Wendt, A Yoshinaga, K AF Watanabe, H. Lorusso, G. Nishimura, S. Xu, Z. Y. Sumikama, T. Soederstroem, P. -A. Doornenbal, P. Browne, F. Gey, G. Jung, H. S. Taprogge, J. Vajta, Zs. Wu, J. Yagi, A. Baba, H. Benzoni, G. Chae, K. Y. Crespi, F. C. L. Fukuda, N. Gernhaeuser, R. Inabe, N. Isobe, T. Jungclaus, A. Kameda, D. Kim, G. D. Kim, Y. K. Kojouharov, I. Kondev, F. G. Kubo, T. Kurz, N. Kwon, Y. K. Lane, G. J. Li, Z. Moon, C. -B. Montaner-Piza, A. Moschner, K. Naqvi, F. Niikura, M. Nishibata, H. Nishimura, D. Odahara, A. Orlandi, R. Patel, Z. Podolyak, Zs. Sakurai, H. Schaffner, H. Simpson, G. S. Steiger, K. Suzuki, H. Takeda, H. Wendt, A. Yoshinaga, K. TI Isomers in Pd-128 and Pd-126: Evidence for a Robust Shell Closure at the Neutron Magic Number 82 in Exotic Palladium Isotopes SO PHYSICAL REVIEW LETTERS LA English DT Article ID NUCLEI; DEFORMATION; SN-100 AB The level structures of the very neutron-rich nuclei Pd-128 and Pd-126 have been investigated for the first time. In the r-process waiting-point nucleus Pd-128, a new isomer with a half-life of 5.8(8) mu s is proposed to have a spin and parity of 8(+) and is associated with a maximally aligned configuration arising from the g(9/2) proton subshell with seniority v = 2. For Pd-126, two new isomers have been identified with half-lives of 0.33(4) and 0.44(3) mu s. The yrast 2(+) energy is much higher in Pd-128 than in Pd-126, while the level sequence below the 8(+) isomer in Pd-128 is similar to that in the N = 82 isotone Cd-130. The electric quadrupole transition that depopulates the 8(+) isomer in Pd-128 is more hindered than the corresponding transition in Cd-130, as expected in the seniority scheme for a semimagic, spherical nucleus. These experimental findings indicate that the shell closure at the neutron number N = 82 is fairly robust in the neutron-rich Pd isotopes. C1 [Watanabe, H.] Beihang Univ, Int Res Ctr Nuclei & Particles Cosmos, Beijing 100191, Peoples R China. [Watanabe, H.] Beihang Univ, Sch Phys & Nucl Energy Engn, Beijing 100191, Peoples R China. [Watanabe, H.; Lorusso, G.; Nishimura, S.; Soederstroem, P. -A.; Doornenbal, P.; Browne, F.; Gey, G.; Taprogge, J.; Vajta, Zs.; Wu, J.; Baba, H.; Fukuda, N.; Inabe, N.; Isobe, T.; Kameda, D.; Kubo, T.; Sakurai, H.; Suzuki, H.; Takeda, H.] RIKEN, Nishina Ctr, Wako, Saitama 3510198, Japan. [Xu, Z. Y.; Niikura, M.] Univ Tokyo, Dept Phys, Bunkyo Ku, Tokyo 1130033, Japan. [Sumikama, T.] Tohoku Univ, Dept Phys, Aoba Ku, Sendai, Miyagi 9808578, Japan. [Browne, F.] Univ Brighton, Sch Comp Engn & Math, Brighton BN2 4GJ, E Sussex, England. [Gey, G.; Simpson, G. S.] Univ Grenoble 1, LPSC, Inst Natl Polytech Grenoble, CNRS IN2P3, F-38026 Grenoble, France. [Jung, H. S.] Chung Ang Univ, Dept Phys, Seoul 156756, South Korea. [Taprogge, J.] Univ Autonoma Madrid, Dept Fis Teor, E-28049 Madrid, Spain. [Taprogge, J.; Jungclaus, A.] CSIC, Inst Estruct Mat, E-28006 Madrid, Spain. [Vajta, Zs.] MTA Atomki, H-4001 Debrecen, Hungary. [Wu, J.; Li, Z.] Peking Univ, Dept Phys, Beijing 100871, Peoples R China. [Yagi, A.; Nishibata, H.; Odahara, A.] Osaka Univ, Dept Phys, Osaka, Toyonaka 5600043, Japan. [Benzoni, G.; Crespi, F. C. L.] INFN, Sez Milano, I-20133 Milan, Italy. [Chae, K. Y.] Sungkyunkwan Univ, Dept Phys, Suwon 440746, South Korea. [Crespi, F. C. L.] Univ Milan, Dipartimento Fis, I-20133 Milan, Italy. [Gernhaeuser, R.; Steiger, K.] Tech Univ Munich, Phys Dept, D-85748 Garching, Germany. [Kim, G. D.; Kim, Y. K.; Kwon, Y. K.] Inst for Basic Sci Korea, Rare Isotope Sci Project, Taejon 305811, South Korea. [Kim, Y. K.] Hanyang Univ, Dept Nucl Engn, Seoul 133791, South Korea. [Kojouharov, I.; Kurz, N.; Schaffner, H.] GSI Helmholtzzentrum Schwerionenforschung GmbH, D-64291 Darmstadt, Germany. [Kondev, F. G.] Argonne Natl Lab, Nucl Engn Div, Argonne, IL 60439 USA. [Lane, G. J.] Australian Natl Univ, Res Sch Phys Sci & Engn, Dept Nucl Phys, Canberra, ACT 0200, Australia. [Moon, C. -B.] Hoseo Univ, Dept Display Engn, Chungnam 336795, South Korea. [Montaner-Piza, A.] Univ Valencia, CSIC, IFIC, E-46071 Valencia, Spain. [Moschner, K.; Wendt, A.] Univ Cologne, Inst Kernphys, D-50937 Cologne, Germany. [Naqvi, F.] Yale Univ, Wright Nucl Struct Lab, New Haven, CT 06520 USA. [Nishimura, D.; Yoshinaga, K.] Tokyo Univ Sci, Fac Sci & Technol, Dept Phys, Noda, Chiba 278, Japan. [Orlandi, R.; Patel, Z.] Katholieke Univ Leuven, Inst Kern Stralingsfys, B-3001 Louvain, Belgium. [Podolyak, Zs.] Univ Surrey, Dept Phys, Guildford GU2 7XH, Surrey, England. RP Watanabe, H (reprint author), Beihang Univ, Int Res Ctr Nuclei & Particles Cosmos, Beijing 100191, Peoples R China. EM hiroshi@ribf.riken.jp RI Lane, Gregory/A-7570-2011; SAKURAI, HIROYOSHI/G-5085-2014 OI Lane, Gregory/0000-0003-2244-182X; FU Rare Isotope Science Project; MSIP; NRF of Korea; Priority Centers Research Program in Korea [2009-0093817]; OTKA [K100835]; U.S. Department of Energy, Office of Nuclear Physics [DE-AC02-06CH11357]; Spanish Ministerio de Ciencia e Innovacion [FPA2009-13377-C02, FPA2011-29854-C04]; JSPS KAKENHI [24740188] FX We are indebted to the facility crews who provided the beams at RIBF, cooperated by RIKEN Nishina Center and CNS, University of Tokyo, the EUROBALL Owners Committee for the loan of germanium detectors, the PreSpec Collaboration for the use of the readout electronics. Part of the WAS3ABi was supported by the Rare Isotope Science Project which is funded by MSIP and NRF of Korea. H. S. J. was supported by the Priority Centers Research Program in Korea (2009-0093817). Zs. V. was supported by OTKA Contract No. K100835. F. G. K. was supported by the U.S. Department of Energy, Office of Nuclear Physics, under Contract No. DE-AC02-06CH11357. We acknowledge financial support from the Spanish Ministerio de Ciencia e Innovacion under Contracts No. FPA2009-13377-C02 and No. FPA2011-29854-C04. We thank Prof. P. Van Isacker, Prof. K. Ogawa, and Dr. Y. Utsuno for valuable discussions and Prof. Y. Gono for warm encouragement. This work was supported by JSPS KAKENHI Grant No. 24740188. NR 28 TC 28 Z9 28 U1 2 U2 24 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 8 PY 2013 VL 111 IS 15 AR 152501 DI 10.1103/PhysRevLett.111.152501 PG 5 WC Physics, Multidisciplinary SC Physics GA 230VX UT WOS:000325372500001 PM 24160593 ER PT J AU Xi, XX Ma, CL Liu, ZX Chen, ZQ Ku, W Berger, H Martin, C Tanner, DB Carr, GL AF Xi, Xiaoxiang Ma, Chunli Liu, Zhenxian Chen, Zhiqiang Ku, Wei Berger, H. Martin, C. Tanner, D. B. Carr, G. L. TI Signatures of a Pressure-Induced Topological Quantum Phase Transition in BiTeI SO PHYSICAL REVIEW LETTERS LA English DT Article ID INSULATOR; SURFACE; STATE; WELLS AB We report the observation of two signatures of a pressure-induced topological quantum phase transition in the polar semiconductor BiTeI using x-ray powder diffraction and infrared spectroscopy. The x-ray data confirm that BiTeI remains in its ambient-pressure structure up to 8 GPa. The lattice parameter ratio c/a shows a minimum between 2.0-2.9 GPa, indicating an enhanced c-axis bonding through p(z) band crossing as expected during the transition. Over the same pressure range, the infrared spectra reveal a maximum in the optical spectral weight of the charge carriers, reflecting the closing and reopening of the semiconducting band gap. Both of these features are characteristics of a topological quantum phase transition and are consistent with a recent theoretical proposal. C1 [Xi, Xiaoxiang; Carr, G. L.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Ma, Chunli; Liu, Zhenxian] Carnegie Inst Sci, Geophys Lab, Washington, DC 20015 USA. [Ma, Chunli] Jilin Univ, State Key Lab Superhard Mat, Changchun 130012, Peoples R China. [Chen, Zhiqiang] SUNY Stony Brook, Dept Geosci, Stony Brook, NY 11794 USA. [Ku, Wei] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Berger, H.] Ecole Polytech Fed Lausanne, Inst Condensed Matter Phys, CH-1015 Lausanne, Switzerland. [Martin, C.; Tanner, D. B.] Univ Florida, Dept Phys, Gainesville, FL 32611 USA. RP Xi, XX (reprint author), Brookhaven Natl Lab, Upton, NY 11973 USA. FU U.S. Department of Energy at BNL [DE-AC02-98CH10886]; NSF (COMPRES) [DMR-0805056, EAR 06-49658]; DOE/NNSA (CDAC) [DE-FC03-03N00144] FX We thank M. S. Bahramy, B.-J. Yang (RIKEN), and Jianming Bai (BNL) for useful discussions. This work was supported by the U.S. Department of Energy through Contract No. DE-AC02-98CH10886 at BNL. The use of U2A and X17C beam lines was supported by NSF (Grants No. DMR-0805056 and No. EAR 06-49658, COMPRES) and DOE/NNSA (Grant No. DE-FC03-03N00144, CDAC). NR 36 TC 59 Z9 59 U1 11 U2 85 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 8 PY 2013 VL 111 IS 15 AR 155701 DI 10.1103/PhysRevLett.111.155701 PG 5 WC Physics, Multidisciplinary SC Physics GA 230VX UT WOS:000325372500005 PM 24160613 ER PT J AU Lumpkin, AH Johnson, AS Ruan, J Thurman-Keup, RM Yao, CY Evtushenko, P AF Lumpkin, A. H. Johnson, A. S. Ruan, J. Thurman-Keup, R. M. Yao, C. -Y. Evtushenko, P. TI Evidence for anomalous optical transition radiation linear polarization effects in beam-profile monitors SO PHYSICAL REVIEW SPECIAL TOPICS-ACCELERATORS AND BEAMS LA English DT Article ID RESOLUTION AB Investigations of the effects of optical transition radiation (OTR) polarization components on beam profiles are presented. The transverse profiles are examined using the OTR perpendicular and parallel polarization components with respect to the dimension of interest. We observed similar to 15% projected profile size reductions with the perpendicularly polarized components on a 65-mu m beam image size case at 14 MeV, a 150-mu m beam image size at 4.5 GeV, and a 1100-mu m beam image size at 7 GeV. These effects are all several times larger than expected (and anomalous in this sense) when compared to the standard OTR point-spread function calculations. We propose the time-averaged induced-current distribution which generates the OTR represents the actual beam size more faithfully with the perpendicular polarization component and recommend its routine use and subsequent deconvolution. C1 [Lumpkin, A. H.; Johnson, A. S.; Ruan, J.; Thurman-Keup, R. M.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Yao, C. -Y.] Argonne Natl Lab, Argonne, IL 60439 USA. [Evtushenko, P.] Thomas Jefferson Natl Lab, Newport News, VA 23606 USA. RP Lumpkin, AH (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. EM lumpkin@fnal.gov FU Fermi Research Alliance, LLC [DE-AC02-07CH11359]; United States Department of Energy; U.S. Department of Energy, Office of Science [DE-ACO2-O6CH11357]; U.S. DOE [DE-AC05-06OR23177, JLAB-BES11-05] FX The authors acknowledge support from N. Eddy and M. Church and the technical assistance of J. Santucci of Fermilab. The first author also acknowledges various discussions on OTR with H. Loos and J. Frisch of SLAC, with R. Ischebeck of PSI, with R. Fiorito of the University of Maryland, and with D. Rule of NSWC. FNAL is operated by Fermi Research Alliance, LLC under Contract No. DE-AC02-07CH11359 with the United States Department of Energy; ANL work was supported by the U.S. Department of Energy, Office of Science, under Contract No. DE-ACO2-O6CH11357; and JLAB contribution was authored by Jefferson Science Associates, LLC under U.S. DOE Contract No. DE-AC05-06OR23177 with modeling and analysis work supported by U. S. DOE office of Basic Energy Sciences under the early career program; DOE Award No. FWP#JLAB-BES11-05. NR 23 TC 0 Z9 0 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-4402 J9 PHYS REV SPEC TOP-AC JI Phys. Rev. Spec. Top.-Accel. Beams PD OCT 8 PY 2013 VL 16 IS 10 AR 102801 DI 10.1103/PhysRevSTAB.16.102801 PG 11 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA 230RK UT WOS:000325359900002 ER PT J AU Kimchi, I Parameswaran, SA Turner, AM Wang, F Vishwanath, A AF Kimchi, Itamar Parameswaran, S. A. Turner, Ari M. Wang, Fa Vishwanath, Ashvin TI Featureless and nonfractionalized Mott insulators on the honeycomb lattice at 1/2 site filling SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article ID INCOMPRESSIBLE QUANTUM FLUID; BOND GROUND-STATES; TOPOLOGICAL ORDER; SUPERFLUID; GAS; ANTIFERROMAGNETS; TRANSITION; MODELS; PHASE AB Within the Landau paradigm, phases of matter are distinguished by spontaneous symmetry breaking. Implicit here is the assumption that a completely symmetric state exists: a paramagnet. At zero temperature such quantum featureless insulators may be forbidden, triggering either conventional order or topological order with fractionalized excitations. Such is the case for interacting particles when the particle number per unit cell, f, is not an integer. However, can lattice symmetries forbid featureless insulators even at integer f? An especially relevant case is the honeycomb (graphene) lattice-where free spinless fermions at f = 1 (the two sites per unit cell mean f = 1 is half-filling per site) are always metallic. Here we present wave functions for bosons, and a related spin-singlet wave function for spinful electrons, on the f = 1 honeycomb lattice and demonstrate via quantum to classical mappings that they do form featureless Mott insulators. The construction generalizes to symmorphic lattices at integer f in any dimension. Our results explicitly demonstrate that in this case, despite the absence of a noninteracting insulator at the same filling, lack of order at zero temperature does not imply fractionalization. C1 [Kimchi, Itamar; Parameswaran, S. A.; Vishwanath, Ashvin] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Turner, Ari M.] Univ Amsterdam, Inst Theoret Phys, NL-1018 XE Amsterdam, Netherlands. [Wang, Fa] Peking Univ, Int Ctr Quantum Mat, Beijing 100871, Peoples R China. [Wang, Fa] Peking Univ, Sch Phys, Beijing 100871, Peoples R China. [Vishwanath, Ashvin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Kimchi, I (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM ikimchi@gmail.com RI Wang, Fa/D-3817-2015 OI Wang, Fa/0000-0002-6220-5349 FU National Science Foundation (NSF) [DGE-1106400, NSF PHY11-25915]; Simons Foundation; Army Research Office; Defense Advanced Research Projects Agency Optical Lattice Emulator program FX We thank Bryan Clark, Matthew Fisher, Tarun Grover, Olexei Motrunich, Shivaji Sondhi, and Matthias Troyer for useful discussions, and Dan Stamper-Kurn and Dan Arovas for collaboration on related work. We also thank an anonymous referee for constructive comments. This research is supported in part by the National Science Foundation (NSF) under Grant DGE-1106400 for the Division of Graduate Education's Graduate Research Fellowship Program and Grant NSF PHY11-25915 for the Kavli Institute for Theoretical Physics Graduate Fellowship Program (I.K.), by the Simons Foundation (S.A.P.), and by the Army Research Office with funding from the Defense Advanced Research Projects Agency Optical Lattice Emulator program (A.V.). NR 37 TC 15 Z9 15 U1 1 U2 9 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD OCT 8 PY 2013 VL 110 IS 41 BP 16378 EP 16383 DI 10.1073/pnas.1307245110 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 231ED UT WOS:000325395600034 ER PT J AU Wang, T Park, YB Caporini, MA Rosay, M Zhong, LH Cosgrove, DJ Hong, M AF Wang, Tuo Park, Yong Bum Caporini, Marc A. Rosay, Melanie Zhong, Linghao Cosgrove, Daniel J. Hong, Mei TI Sensitivity-enhanced solid-state NMR detection of expansin's target in plant cell walls SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE carbohydrate-binding module; CBM ID DYNAMIC NUCLEAR-POLARIZATION; SPIN-LATTICE-RELAXATION; BACTERIAL EXPANSIN; CRYSTAL-STRUCTURE; CELLULOSE; XYLOGLUCAN; POLYSACCHARIDES; SPECTROSCOPY; ARABIDOPSIS; BINDING AB Structure determination of protein binding to noncrystalline macromolecular assemblies such as plant cell walls (CWs) poses a significant structural biology challenge. CWs are loosened during growth by expansin proteins, which weaken the noncovalent network formed by cellulose, hemicellulose, and pectins, but the CW target of expansins has remained elusive because of the minute amount of the protein required for activity and the complex nature of the CW. Using solid-state NMR spectroscopy, combined with sensitivity-enhancing dynamic nuclear polarization (DNP) and differential isotopic labeling of expansin and polysaccharides, we have now determined the functional binding target of expansin in the Arabidopsis thaliana CW. By transferring the electron polarization of a biradical dopant to the nuclei, DNP allowed selective detection of C-13 spin diffusion from trace concentrations of C-13, N-15-labeled expansin in the CW to nearby polysaccharides. From the spin diffusion data of wild-type and mutant expansins, we conclude that to loosen the CW, expansin binds highly specific cellulose domains enriched in xyloglucan, whereas more abundant binding to pectins is unrelated to activity. Molecular dynamics simulations indicate short C-13-C-13 distances of 4-6 angstrom between a hydrophobic surface of the cellulose microfibril and an aromatic motif on the expansin surface, consistent with the observed NMR signals. DNP-enhanced 2D C-13 correlation spectra further reveal that the expansin-bound cellulose has altered conformation and is enriched in xyloglucan, thus providing unique insight into the mechanism of CW loosening. DNP-enhanced NMR provides a powerful, generalizable approach for investigating protein binding to complex macromolecular targets. C1 [Wang, Tuo; Hong, Mei] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. [Wang, Tuo; Hong, Mei] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. [Park, Yong Bum; Cosgrove, Daniel J.] Penn State Univ, Dept Biol, University Pk, PA 16802 USA. [Caporini, Marc A.; Rosay, Melanie] Bruker Biospin Corp, Billerica, MA 01821 USA. [Zhong, Linghao] Penn State Univ, Dept Chem, Mt Alto, PA 17237 USA. RP Cosgrove, DJ (reprint author), Penn State Univ, Dept Biol, University Pk, PA 16802 USA. EM dcosgrove@psu.edu; mhong@iastate.edu FU Department of Energy (DOE) [AL 10-501-117163]; DOE-Basic Energy Science (BES) [DE-FG02-84ER13179]; US-DOE-BES-Energy Frontier Research Centers Award [DE-SC0001090] FX We thank Edward Wagner for help in producing labeled protein. T.W. and M.H. acknowledge Department of Energy (DOE) Grant AL 10-501-117163, D.J.C. and L.Z. acknowledge DOE-Basic Energy Science (BES) Grant DE-FG02-84ER13179, and Y.B.P. was supported by US-DOE-BES-Energy Frontier Research Centers Award DE-SC0001090. NR 45 TC 69 Z9 71 U1 5 U2 115 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD OCT 8 PY 2013 VL 110 IS 41 BP 16444 EP 16449 DI 10.1073/pnas.1316290110 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 231ED UT WOS:000325395600045 PM 24065828 ER PT J AU Boudreau, A Tanner, K Wang, D Geyer, FC Reis-Filho, JS Bissell, MJ AF Boudreau, Aaron Tanner, Kandice Wang, Daojing Geyer, Felipe C. Reis-Filho, Jorge S. Bissell, Mina J. TI 14-3-3 sigma stabilizes a complex of soluble actin and intermediate filament to enable breast tumor invasion SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE cytoskeleton; motility; 14-3-3 family; triple-negative; basal breast cancer ID GENE-EXPRESSION SIGNATURE; EPITHELIAL-CELLS; SACCHAROMYCES-CEREVISIAE; XENOGRAFT MODEL; IN-SITU; CANCER; PROTEINS; PROGRESSION; STRESS; CYTOSKELETON AB The protein 14-3-3s (stratifin) is frequently described as a tumor suppressor silenced in about 80% of breast tumors. Intriguingly, we show that 14-3-3s expression, which in normal breast is localized to the myoepithelial cells, tracks with malignant phenotype in two models of basal-like breast cancer progression, and in patients, it is associated with basal-like subtype and poor clinical outcome. We characterized a mechanism by which 14-3-3s guides breast tumor invasion by integrating cytoskeletal dynamics: it stabilizes a complex of solubilized actin and intermediate filaments to maintain a pool of "bioavailable"complexes for polarized assembly during migration. We show that formation of the actin/cytokeratin/ 14-3-3s complex and cellular migration are regulated by PKC.dependent phosphorylation, a finding that could form the basis for intervention in aggressive breast carcinomas expressing 14-33s. Our data suggest that the biology of this protein is important in cellular movement and is contingent on breast cancer subtype. C1 [Boudreau, Aaron; Tanner, Kandice; Wang, Daojing; Bissell, Mina J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Life Sci Div, Berkeley, CA 94720 USA. [Geyer, Felipe C.; Reis-Filho, Jorge S.] Inst Canc Res, Mol Pathol Lab, Breakthrough Breast Canc Res Ctr, London SW3 6JB, England. RP Boudreau, A (reprint author), Univ Calif San Francisco, Dept Lab Med, San Francisco, CA 94115 USA. EM atboudreau@lbl.gov; mjbissell@lbl.gov FU Department of Defense Predoctoral Fellowship [W81XWH-051-0339]; California Breast Cancer Research Program Dissertation [14GB-0007]; Breakthrough Breast Cancer; US Department of Energy Low Dose Radiation Research Program; US Department of Energy Office of Biological and Environmental Research; Low Dose Radiation Program [DE-AC02-05CH1123]; National Cancer Institute [R37CA064786, R01CA140663, U54CA112970, U01CA143233, U54CA143836]; Bay Area Physical Sciences-Oncology Center (University of California, Berkeley); US Department of Defense [W81XWH0810736]; Breast Cancer Research Foundation FX We thank Genee Lee, Connie Myers, Aylin Rizki, Paraic Kenny, Britta Weigelt, Jason Jung, Joe Gray, Marc Lenburg, Eric Collisson, Sanjay Kumar, Laura van 't Veer, and all members of the M.J.B. laboratory for either excellent technical advice and/or fruitful discussions. We also thank Roland Meier for generously helping with xenograft experiments and Kay Savage for help in scoring the tissue microarrays. This work was funded by Department of Defense Predoctoral Fellowship W81XWH-051-0339 and California Breast Cancer Research Program Dissertation Award 14GB-0007 (to A.B.). For this work, J.S.R.-F. and F.C.G. were funded, in part, by Breakthrough Breast Cancer. D.W. received funding support from the US Department of Energy Low Dose Radiation Research Program. The work of the M. J.B. laboratory is supported by grants from the US Department of Energy Office of Biological and Environmental Research and the Low Dose Radiation Program (Contract DE-AC02-05CH1123); by National Cancer Institute Grants R37CA064786, R01CA140663, U54CA112970, U01CA143233, and U54CA143836 awarded to the Bay Area Physical Sciences-Oncology Center (University of California, Berkeley); by US Department of Defense Grant W81XWH0810736; and, in part, by a grant from The Breast Cancer Research Foundation. NR 54 TC 15 Z9 15 U1 1 U2 19 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD OCT 8 PY 2013 VL 110 IS 41 BP E3937 EP E3944 DI 10.1073/pnas.1315022110 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 231ED UT WOS:000325395600010 PM 24067649 ER PT J AU Wittke, JH Bunch, TE Kennett, JP Kennett, DJ Culleton, BJ Tankersley, KB Daniel, IR Kloosterman, JB Kletetschka, G West, A Firestone, RB AF Wittke, James H. Bunch, Ted E. Kennett, James P. Kennett, Douglas J. Culleton, Brendan J. Tankersley, Kenneth B. Daniel, I. Randolph, Jr. Kloosterman, Johan B. Kletetschka, Gunther West, Allen Firestone, Richard B. TI Reply to van Hoesel et al.: Impact-related Younger Dryas boundary nanodiamonds from The Netherlands SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Letter C1 [Wittke, James H.; Bunch, Ted E.] No Arizona Univ, Sch Earth Sci & Environm Sustainabil, Dept Geol, Flagstaff, AZ 86011 USA. [Kennett, James P.] Univ Calif Santa Barbara, Inst Marine Sci, Dept Earth Sci, Santa Barbara, CA 93106 USA. [Kennett, Douglas J.; Culleton, Brendan J.] Penn State Univ, Dept Anthropol, University Pk, PA 16802 USA. [Tankersley, Kenneth B.] Univ Cincinnati, Dept Anthropol, Cincinnati, OH 45221 USA. [Tankersley, Kenneth B.] Univ Cincinnati, Dept Geol, Cincinnati, OH 45221 USA. [Daniel, I. Randolph, Jr.] E Carolina Univ, Dept Anthropol, Greenville, NC 27858 USA. [Kloosterman, Johan B.] Explorat Geologist, NL-1016 NN Amsterdam, Netherlands. [Kletetschka, Gunther] Charles Univ Prague, Fac Sci, Prague 12843, Czech Republic. [Kletetschka, Gunther] Acad Sci Czech Republic, Inst Geol, Prague 16500, Czech Republic. [West, Allen] GeoSci Consulting, Dewey, AZ 86327 USA. [Firestone, Richard B.] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Bunch, TE (reprint author), No Arizona Univ, Sch Earth Sci & Environm Sustainabil, Dept Geol, Flagstaff, AZ 86011 USA. EM tbear1@cableone.net RI Kletetschka, Gunther/C-9996-2011; Kennett, Douglas/I-7613-2015; OI Kletetschka, Gunther/0000-0002-0645-9037; Kennett, Douglas/0000-0001-5133-9010; Firestone, Richard/0000-0003-3833-5546 NR 6 TC 2 Z9 2 U1 0 U2 22 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD OCT 8 PY 2013 VL 110 IS 41 BP E3897 EP E3898 DI 10.1073/pnas.1313207110 PG 2 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 231ED UT WOS:000325395600003 PM 24244962 ER PT J AU Wittke, JH Bunch, TE Tankersley, KB Daniel, IR Kloosterman, JB Kletetschka, G West, A Firestone, RB AF Wittke, James H. Bunch, Ted E. Tankersley, Kenneth B. Daniel, I. Randolph, Jr. Kloosterman, Johan B. Kletetschka, Gunther West, Allen Firestone, Richard B. TI Reply to Ives and Froese: Regarding the impact-related Younger Dryas boundary layer at Chobot site, Alberta, Canada SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Letter C1 [Wittke, James H.; Bunch, Ted E.] No Arizona Univ, Sch Earth Sci & Environm Sustainabil, Geol Program, Flagstaff, AZ 86011 USA. [Tankersley, Kenneth B.] Univ Cincinnati, Dept Anthropol & Geol, Cincinnati, OH 45221 USA. [Daniel, I. Randolph, Jr.] E Carolina Univ, Dept Anthropol, Greenville, NC 27858 USA. [Kloosterman, Johan B.] Explorat Geologist, NL-1016 NN Amsterdam, Netherlands. [Kletetschka, Gunther] Charles Univ Prague, Fac Sci, Prague 12843, Czech Republic. [Kletetschka, Gunther] Acad Sci Czech Republic, Inst Geol, Prague 16500, Czech Republic. [West, Allen] GeoSci Consulting, Dewey, AZ USA. Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Bunch, TE (reprint author), No Arizona Univ, Sch Earth Sci & Environm Sustainabil, Geol Program, Flagstaff, AZ 86011 USA. EM tbear1@cableone.net RI Kletetschka, Gunther/C-9996-2011; OI Kletetschka, Gunther/0000-0002-0645-9037; Firestone, Richard/0000-0003-3833-5546 NR 5 TC 2 Z9 2 U1 1 U2 21 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD OCT 8 PY 2013 VL 110 IS 41 BP E3900 EP E3900 DI 10.1073/pnas.1313408110 PG 1 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 231ED UT WOS:000325395600005 PM 24244963 ER PT J AU Bell, MJ Beck, AR Mashiko, H Neumark, DM Leone, SR AF Bell, M. Justine Beck, Annelise R. Mashiko, Hiroki Neumark, Daniel M. Leone, Stephen R. TI Intensity dependence of light-induced states in transient absorption of laser-dressed helium measured with isolated attosecond pulses SO JOURNAL OF MODERN OPTICS LA English DT Article DE ultrafast optics; attosecond spectroscopy; dressed absorption; XUV ID REAL-TIME OBSERVATION; EXTREME-ULTRAVIOLET; QUANTUM DYNAMICS; ELECTRIC-FIELD; SPECTROSCOPY; FEMTOSECOND; EXCITATION; ATOMS; NM AB Light-induced states in He atoms were characterized using attosecond transient absorption spectroscopy. A 400 as pulse covering the 20-24eV spectral range serves as the probe pulse, and the effect of a few-cycle near infrared pulse (12 fs, 780nm) on the absorption spectrum is measured as a function of time delay and near-infrared intensities varying from (5.0 +/- 2)x10(10) to (1 +/- 0.4)x10(13)W/cm(2). Light-induced states resulting from near-infrared coupling of 1s2p to 1s2s, 1s3d, and 1s3s states are observed. Absorption features that likely result from coupling of 1s3p to 1s4s, 1s4d, 1s5s, and 1s5d states are also observed. The light-induced states with the smallest detunings (1s3d and 1s3s) from the dressing frequency may shift to higher frequencies as the dressing intensity is increased. C1 [Bell, M. Justine; Beck, Annelise R.; Mashiko, Hiroki; Neumark, Daniel M.; Leone, Stephen R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Bell, M. Justine; Beck, Annelise R.; Mashiko, Hiroki; Neumark, Daniel M.; Leone, Stephen R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Leone, Stephen R.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. RP Neumark, DM (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM dneumark@berkeley.edu; srl@berkeley.edu FU Division of Chemical Sciences, Geosciences, and Biosciences of the U.S. Department of Energy at LBNL [DE-AC02-05CH11231]; NSF-GRFP; National Security Science and Engineering Faculty Fellowship FX This work was supported by the Director, Office of Science, Office of Basic Energy Sciences, and by the Division of Chemical Sciences, Geosciences, and Biosciences of the U.S. Department of Energy at LBNL under Contract No. DE-AC02-05CH11231. M.J.B. and A. R. B. acknowledge funding from NSF-GRFP. S. R. L acknowledges the support of a National Security Science and Engineering Faculty Fellowship. T. Pfeiffer, A.N. Pfeiffer are thanked for helpful discussions of experimental details. NR 39 TC 11 Z9 11 U1 2 U2 26 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND SN 0950-0340 EI 1362-3044 J9 J MOD OPTIC JI J. Mod. Opt. PD OCT 7 PY 2013 VL 60 IS 17 SI SI BP 1506 EP 1516 DI 10.1080/09500340.2013.826389 PG 11 WC Optics SC Optics GA 269MQ UT WOS:000328245800014 ER PT J AU Pereira, CCL Maurice, R Lucena, AF Hu, SX Goncalves, AP Marcalo, J Gibson, JK Andrews, L Gagliardi, L AF Pereira, Claudia C. L. Maurice, Remi Lucena, Ana F. Hu, Shuxian Goncalves, Antonio P. Marcalo, Joaquim Gibson, John K. Andrews, Lester Gagliardi, Laura TI Thorium and Uranium Carbide Cluster Cations in the Gas Phase: Similarities and Differences between Thorium and Uranium SO INORGANIC CHEMISTRY LA English DT Article ID ABLATION MASS-SPECTROMETRY; TRANSITION-METAL COMPOUNDS; LASER-ABLATION; THERMODYNAMIC PROPERTIES; ELECTRON LOCALIZATION; PREDICTED STABILITY; MOLECULAR-STRUCTURE; ION FORMATION; BASIS-SETS; DICARBIDE AB Laser ionization of AnC(4) alloys (An = Th, U) yielded gas-phase molecular thorium and uranium carbide cluster cations of composition An(m)C(n)(+), with m = 1, n = 2-14, and m = 2, n = 3-18, as detected by Fourier transform ion-cyclotron-resonance mass spectrometry. In the case of thorium, ThmCn+ cluster ions with m = 3-13 and n = 5-30 were also produced, with an intriguing high intensity of Th13Cn+ cations. The AnC(13)(+) ions also exhibited an unexpectedly high abundance, in contrast to the gradual decrease in the intensity of other AnC(n)(+) ions with increasing values of n. High abundances of AnC(2)(+) and AnC(4)(+) ions are consistent with enhanced stability due to strong metal-C-2 bonds. Among the most abundant bimetallic ions was Th2C3+ for thorium; in contrast, U2C4+ was the most intense bimetallic for uranium, with essentially no U2C3+ appearing. Density functional theory computations were performed to illuminate this distinction between thorium and uranium. The computational results revealed structural and energetic isparities for the An(2)C(3)(+) and An(2)C(4)(+) cluster ions, which elucidate the observed differing abundances of the bimetallic carbide ions. Particularly noteworthy is that the Th atoms are essentially equivalent in Th2C3+, whereas there is a large asymmetry between the U atoms in U2C3+. C1 [Pereira, Claudia C. L.; Lucena, Ana F.; Goncalves, Antonio P.; Marcalo, Joaquim] Univ Tecn Lisboa, Inst Super Tecn, IST ITN, Unidade Ciencias Quim & Radiofarmaceut, P-2686953 Sacavem, Portugal. [Maurice, Remi; Hu, Shuxian; Gagliardi, Laura] Univ Minnesota, Dept Chem, Inst Supercomp, Minneapolis, MN 55455 USA. [Maurice, Remi; Hu, Shuxian; Gagliardi, Laura] Univ Minnesota, Chem Theory Ctr, Minneapolis, MN 55455 USA. [Gibson, John K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Andrews, Lester] Univ Virginia, Dept Chem, Charlottesville, VA 22904 USA. RP Marcalo, J (reprint author), Univ Tecn Lisboa, Inst Super Tecn, IST ITN, Unidade Ciencias Quim & Radiofarmaceut, P-2686953 Sacavem, Portugal. EM jmarcalo@ctn.ist.utl.pt; gagliard@umn.edu RI PTMS, RNEM/C-1589-2014; Marcalo, Joaquim/J-5476-2013; Pereira Goncalves, Antonio/B-2849-2008; OI Marcalo, Joaquim/0000-0001-7580-057X; Pereira Goncalves, Antonio/0000-0003-2640-3038; Pereira, Claudia/0000-0003-3421-8676 FU Fundacao para a Ciencia e a Tecnologia/Portugal [SFRH/BD/70475/2010]; Office of Basic Energy Sciences, U.S. Department of Energy [USDOE/DESC002183]; U.S. Department of Energy, Office of Basic Energy Sciences, Heavy Element Chemistry, at LBNL [DE-AC02-05CH11231] FX R.M. thanks David Semrouni for helpful discussions. The authors are grateful to Fundacao para a Ciencia e a Tecnologia/Portugal ("Ciencia 2007" Programme; Ph.D. Grant SFRH/BD/70475/2010 to A.F.L.). The work by R.M., S.H. and L.G. was supported by the Director, Office of Basic Energy Sciences, U.S. Department of Energy, under Contract USDOE/DESC002183. The work by J.K.G. was fully supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Heavy Element Chemistry, at LBNL under Contract DE-AC02-05CH11231. NR 56 TC 5 Z9 5 U1 4 U2 50 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD OCT 7 PY 2013 VL 52 IS 19 BP 10968 EP 10975 DI 10.1021/ic401058b PG 8 WC Chemistry, Inorganic & Nuclear SC Chemistry GA 243MF UT WOS:000326319800038 PM 24047411 ER PT J AU Odoh, SO Govind, N Schreckenbach, G de Jong, WA AF Odoh, Samuel O. Govind, Niranjan Schreckenbach, Georg de Jong, Wibe A. TI Cation-Cation Interactions in [(UO2)(2)(OH)(n)](4-n) Complexes SO INORGANIC CHEMISTRY LA English DT Article ID DENSITY-FUNCTIONAL CALCULATIONS; GAS-PHASE CHEMISTRY; EFFECTIVE CORE POTENTIALS; MATRIX INFRARED-SPECTRA; URANYL-ION; URANIUM ATOMS; SOLID ARGON; ELECTRONIC-STRUCTURES; CRYSTAL-STRUCTURE; LIGAND-EXCHANGE AB The structures and bonding of gas-phase [(UO2)(2)(OH)(n)](4-n) (n = 2-6) complexes have been studied using density functional theory (DFT), MP2, and CCSD(T) methods with particular emphasis on ground state structures featuring cation-cation interactions (CCIs) between the uranyl groups. An interesting trend is observed in the stabilities of members of this series of complexes. The structures of [(UO2)(2)(OH)(2)](2+), [(UO2)(2)(OH)(4)], and [(UO2)(2)(OH)(6)](2-) featuring CCIs are found at higher energies (by 3-27 kcal/mol) in comparison to their conventional mu(2)-dihydroxo structures. In contrast, the CCI structures of [(UO2)(2)(OH)(3)](+) and [(UO2)(2)(OH)(5)](-) are respectively degenerate with and lower in energy than the structures with the mu(2)-dihydroxo format. The origin of this trend lies in the symmetry-based need to balance the coordination numbers and effective atomic charges of each uranium center. The calculated IR vibrational frequencies provide signature probes that can be used in differentiating the low-energy structures and in experimentally confirming the existence of the structures featuring CCIs. C1 [Odoh, Samuel O.; Govind, Niranjan; de Jong, Wibe A.] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Schreckenbach, Georg] Univ Manitoba, Dept Chem, Winnipeg, MB R3T 2N2, Canada. RP de Jong, WA (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM wibe.dejong@pnnl.gov RI DE JONG, WIBE/A-5443-2008 OI DE JONG, WIBE/0000-0002-7114-8315 FU BES Heavy Element Chemistry program in the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy; Natural Sciences and Engineering Research Council of Canada (NSERC); U.S. Department of Energy's Office of Biological and Environmental Research FX This research was funded by the BES Heavy Element Chemistry program in the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy. G.S. acknowledges financial support from the Natural Sciences and Engineering Research Council of Canada (NSERC). All calculations were performed using the Molecular Science Computing Capability in the William R. Wiley Environmental Molecular Science Laboratory, a national scientific user facility sponsored by the U.S. Department of Energy's Office of Biological and Environmental Research and located at the Pacific Northwest National Laboratory, operated for the Department of Energy by Battelle. NR 93 TC 3 Z9 3 U1 4 U2 35 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD OCT 7 PY 2013 VL 52 IS 19 BP 11269 EP 11279 DI 10.1021/ic4015338 PG 11 WC Chemistry, Inorganic & Nuclear SC Chemistry GA 243MF UT WOS:000326319800069 PM 24024761 ER PT J AU Peng, Q Li, M Hu, CJ Pavlik, JW Oliver, AG Alp, EE Hu, MY Zhao, JY Sage, JT Scheidt, WR AF Peng, Qian Li, Ming Hu, Chuanjiang Pavlik, Jeffrey W. Oliver, Allen G. Alp, E. Ercan Hu, Michael Y. Zhao, Jiyong Sage, J. Timothy Scheidt, W. Robert TI Probing Heme Vibrational Anisotropy: An Imidazole Orientation Effect? SO INORGANIC CHEMISTRY LA English DT Article ID AXIAL LIGAND ORIENTATION; ELECTRON-PARAMAGNETIC-RES; NUCLEAR RESONANT SCATTERING; MAIN-GROUP THERMOCHEMISTRY; HINDERED PORPHYRIN SYSTEM; SPIN FERRIC PORPHYRINS; JAHN-TELLER DISTORTION; DENSITY-OF-STATES; MOLECULAR-STRUCTURE; CYTOCHROMES-B AB The complete iron vibrational spectrum of the five-coordinate high-spin complex [Fe(OEP)(2-MeHIm)], where OEP = octaethylporphyrinato and 2-MeHIM = 2-methylimidazole, has been obtained by oriented single-crystal nuclear resonance vibrational spectroscopy (NRVS) data. Measurements have been made in three orthogonal directions, which provides quantitative information for all iron motion. These experimental data, buttressed by density functional theory (DFT) calculations, have been used to define the effects of the axial ligand orientation. Although the axial imidazole removes the degeneracy in the in-plane vibrations, the imidazole orientation does not appear to control the direction of the in-plane iron motion. This is in contrast to the effect of the imidazolate ligand, as defined by DFT calculations, which does have substantial effects on the direction of the in-plane iron motion. The axial NO ligand has been found to have the strongest orientational effect (Angew. Chem., Int. Ed., 2010, 49, 4400). Thus the strength of the directional properties are in the order NO > imidazolate > imidazole, consistent with the varying strength of the Fe-ligand bond. C1 [Peng, Qian; Li, Ming; Hu, Chuanjiang; Pavlik, Jeffrey W.; Oliver, Allen G.; Scheidt, W. Robert] Univ Notre Dame, Dept Chem & Biochem, Notre Dame, IN 46556 USA. [Hu, Chuanjiang] Soochow Univ, Coll Chem Chem Engn & Mat Sci, Key Lab Organ Synth Jiangsu Prov, Suzhou 215123, Peoples R China. [Alp, E. Ercan; Hu, Michael Y.; Zhao, Jiyong] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Sage, J. Timothy] Northeastern Univ, Dept Phys, Boston, MA 02115 USA. [Sage, J. Timothy] Northeastern Univ, Ctr Interdisciplinary Res Complex Syst, Boston, MA 02115 USA. RP Sage, JT (reprint author), Northeastern Univ, Dept Phys, Boston, MA 02115 USA. EM jtsage@neu.edu; scheidt.1@nd.edu RI Peng, Qian/N-7093-2013 OI Peng, Qian/0000-0002-1218-5976 FU National Institutes of Health [GM-38401]; National Natural Science Foundation of China [21271133]; NSF [CHE-1026369]; U.S. DOE [DE-AC02-06CH11357] FX We thank the National Institutes of Health for support of this research under Grant GM-38401 to W.R.S., the National Natural Science Foundation of China (No. 21271133) for support of this research to C.H., and the NSF under CHE-1026369 to J.T.S. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No, DE-AC02-06CH11357. We thank Lili Gao for assistance with NRVS data reduction. NR 89 TC 3 Z9 3 U1 1 U2 23 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD OCT 7 PY 2013 VL 52 IS 19 BP 11361 EP 11369 DI 10.1021/ic401644g PG 9 WC Chemistry, Inorganic & Nuclear SC Chemistry GA 243MF UT WOS:000326319800079 PM 24020589 ER PT J AU Bera, TK Iyer, RG Malliakas, CD Kanatzidis, MG AF Bera, Tarun K. Iyer, Ratnasabapathy G. Malliakas, Christos D. Kanatzidis, Mercouri G. TI Crystalline and Glassy Phases in the Cs/Bi/As/S System SO INORGANIC CHEMISTRY LA English DT Article ID STRONG 2ND-HARMONIC GENERATION; BAND-GAP SEMICONDUCTORS; CHALCOGENIDE GLASS; QUATERNARY BISMUTH; BUILDING-BLOCKS; RB; CS; AS2S3; SE; NA AB The quaternary Cs2S/Bi/As/S system was studied in an attempt to introduce two different asymmetric but isoelectronic building units, namely, [(BixSy)-S-III] and [(AsxSy)-S-III], in a single structure. Reactions with a comparatively lower equivalent of arsenic in the Cs2S/Bi/As/S mixture led to the crystalline compound Cs3Bi(AsS4)(2). The structure features tetrahedral [(AsS4)-S-V](3-) connected to Bi-III centers to give infinite 1/infinity[Bi(AsS4)(2)(3-)] chains. When the basicity was raised in these low arsenic fluxes by increasing the Cs2S fraction, the crystalline compound Cs9Bi(AsS4)(4), also featuring [(AsS4)-S-V](3-) anions, was formed. On the other hand, arsenic-rich mixtures of Cs2S/Bi/As/S led to the formation of the glassy phase Cs2BiAs3S7, which contains As-III species. X-ray photoelectron spectroscopy (XPS), Raman spectroscopy, and pair distribution function (PDF) analysis indicate the presence of As-III-containing [AsnS2n+1] fragments in the glass structure. Several glasses in the series Csn-1BiAsnS2n+1 were also prepared using solid-state fusion reactions. The band gaps of the Csn-1BiAsnS2n+1 glasses are in the range of 1.51-1.81 eV, while that of the crystalline compound Cs3Bi(AsS4)(2) is similar to 2.33 eV. The thermal and optical behaviors of these compounds are correlated with their structures and building units. C1 [Bera, Tarun K.; Malliakas, Christos D.; Kanatzidis, Mercouri G.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Kanatzidis, Mercouri G.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Iyer, Ratnasabapathy G.] Claflin Univ, Dept Chem, Orangeburg, SC 29118 USA. RP Kanatzidis, MG (reprint author), Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. EM m-kanatzidis@northwestern.edu FU National Science Foundation [DMR-1104965]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE4-AC02406CH11357] FX Financial support from the National Science Foundation (Grant DMR-1104965) is gratefully acknowledged. This work made use of the SEM facilities at the Electron Probe Instrumentation Center, Northwestern University. The FT-Raman spectroscopic study was done at the Analytical Service Laboratory, Northwestern University. Use of the Advanced Photon Source at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE4-AC02406CH11357. NR 53 TC 2 Z9 2 U1 2 U2 29 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD OCT 7 PY 2013 VL 52 IS 19 BP 11370 EP 11376 DI 10.1021/ic4016542 PG 7 WC Chemistry, Inorganic & Nuclear SC Chemistry GA 243MF UT WOS:000326319800080 PM 24063370 ER PT J AU Laurita, G Page, K Sleight, AW Subramanian, MA AF Laurita, Geneva Page, Katharine Sleight, A. W. Subramanian, M. A. TI Structural Investigation of the Substituted Pyrochlore AgSbO3 through Total Scattering Techniques SO INORGANIC CHEMISTRY LA English DT Article ID THERMOELECTRIC PROPERTIES; LIGHT IRRADIATION; OXIDES; PEROVSKITE AB Polycrystalline samples of the pyrochlore series (Ag1-xMxSbO3+x[(n-1)/2])-Sb-n (M = Na, K, and Tl) have been structurally analyzed through total scattering techniques. The upper limits of x obtained were 0.05 for Na, 0.16 for K, and 0.17 for Tl. The Ag+ cation occupies a site with inversion symmetry on a 3-fold axis. When the smaller Na+ cation substitutes for Ag+, it is displaced by about 0.6 angstrom perpendicular to the 3-fold axis to achieve some shorter Na-O bond distances. When the larger Tl+ cation substitutes for Ag+, it is displaced by about 1.14 angstrom along the 3-fold axis and achieves an environment typical of a lone pair cation. Some of the Tl3+ from the precursor remains unreduced, leading to a formula of Ag0.772(1)Tl0.13(2)+Tl0.036(1)3+SbO3.036(1). The position of the K+ dopant was effectively modeled assuming that K+ occupied the same site as Ag+. The expansion of the lattice caused by substitution of the larger K+ and Tl+ cations results in longer Ag-O bond lengths, which would reduce the overlap of the Ag 4d and O 2p orbitals that compose the valence band maximum. Substitution of the smaller Na+ results in a decrease in the Ag O bond distance, thus increasing the overlap of the Ag 4d and O 2p orbitals. This will have a direct influence on the band composition and observed properties of this material of interest. C1 [Laurita, Geneva; Sleight, A. W.; Subramanian, M. A.] Oregon State Univ, Dept Chem, Corvallis, OR 97331 USA. [Page, Katharine] Los Alamos Natl Lab, Lujan Neutron Scattering Ctr, LANSCE LC, Los Alamos, NM 87545 USA. RP Subramanian, MA (reprint author), Oregon State Univ, Dept Chem, Gilbert Hall 153, Corvallis, OR 97331 USA. EM mas.subramanian@oregonstate.edu RI Page, Katharine/C-9726-2009 OI Page, Katharine/0000-0002-9071-3383 FU NSF [CHE-1102637]; DoE BES; DoE [DEAC52-06NA25396]; National Science Foundation [DMR 00-76488] FX This work was supported by NSF Grant CHE-1102637. We thank Joan Siewenie at Los Alamos National Laboratory for her assistance with the neutron data collection and reduction, and Dr. Jun Li for her helpful discussions in regards to Rietveld analysis. This work benefitted from the use of NPDF at the Lujan Center at Los Alamos Neutron Science Center, funded by DoE BES. Los Alamos National Laboratory is operated by Los Alamos National Security LLC under DoE Contract DEAC52-06NA25396. The upgrade of NPDF was funded by the National Science Foundation through Grant DMR 00-76488. NR 26 TC 2 Z9 2 U1 1 U2 19 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD OCT 7 PY 2013 VL 52 IS 19 BP 11530 EP 11537 DI 10.1021/ic401860j PG 8 WC Chemistry, Inorganic & Nuclear SC Chemistry GA 243MF UT WOS:000326319800097 PM 24020701 ER PT J AU Bogart, JA Lewis, AJ Medling, SA Piro, NA Carroll, PJ Booth, CH Schelter, EJ AF Bogart, Justin A. Lewis, Andrew J. Medling, Scott A. Piro, Nicholas A. Carroll, Patrick J. Booth, Corwin H. Schelter, Eric J. TI Homoleptic Cerium(III) and Cerium(IV) Nitroxide Complexes: Significant Stabilization of the 4+Oxidation State SO INORGANIC CHEMISTRY LA English DT Article ID GAS SHIFT REACTION; OXIDE FUEL-CELLS; OXIDATION-STATES; LANTHANIDE CHEMISTRY; MAGNETIC-PROPERTIES; TRANSITION-METAL; CERIA; LIGAND; CATALYSTS; NITRIDE AB Electrochemical experiments performed on the complex Ce-IV[2-((BuNO)-Bu-t)py](4), where [2-((BuNO)-Bu-t)py](-) = N-tert-butyl-N-2-pyridylnitroxide, indicate a 2.51 V stabilization of the 4+ oxidation state of Ce compared to [(Bu4N)-Bu-n](2)[Ce(NO3)(6)] in acetonitrile and a 2.95 V stabilization compared to the standard potential for the ion under aqueous conditions. Density functional theory calculations suggest that this preference for the higher oxidation state is a result of the tetrakis(nitroxide) ligand framework at the Ce cation, which allows for effective electron donation into, and partial covalent overlap with, vacant 4f orbitals with delta symmetry. The results speak to the behavior of CeO2 and related solid solutions in oxygen uptake and transport applications, in particular an inherent local character of bonding that stabilizes the 4+ oxidation state. The results indicate a cerium(IV) complex that has been stabilized to an unprecedented degree through tuning of its ligand-field environment. C1 [Bogart, Justin A.; Lewis, Andrew J.; Piro, Nicholas A.; Carroll, Patrick J.; Schelter, Eric J.] Univ Penn, Dept Chem, P Roy & Diana T Vagelos Labs, Dept Chem, Philadelphia, PA 19104 USA. [Medling, Scott A.; Booth, Corwin H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Schelter, EJ (reprint author), Univ Penn, Dept Chem, P Roy & Diana T Vagelos Labs, Dept Chem, Philadelphia, PA 19104 USA. EM schelter@sas.upenn.edu FU U.S. Department of Energy, Office of Science, Early Career Research Program [DE-SC0006518]; University of Pennsylvania; National Science Foundation [OCI-1053575]; Office of Science (OS), Office of Basic Energy Sciences, of the U.S. Department of Energy (DOE) [DE-AC02-05CH11231] FX E.J.S. acknowledges the U.S. Department of Energy, Office of Science, Early Career Research Program (Grant DE-SC0006518), and the University of Pennsylvania for financial support of this work. We thank Prof. Raymond J. Gorte, University of Pennsylvania, for helpful discussion. This work used the Extreme Science and Engineering Discovery Environment (XSEDE), which is supported by National Science Foundation Grant OCI-1053575. Portions of this work were supported by the Director, Office of Science (OS), Office of Basic Energy Sciences, of the U.S. Department of Energy (DOE) under Contract DE-AC02-05CH11231 and were carried out at SSRL, a Directorate of SLAC National Accelerator Laboratory and an OS User Facility operated for the DOE OS by Stanford University. NR 69 TC 26 Z9 26 U1 0 U2 35 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD OCT 7 PY 2013 VL 52 IS 19 BP 11600 EP 11607 DI 10.1021/ic401974t PG 8 WC Chemistry, Inorganic & Nuclear SC Chemistry GA 243MF UT WOS:000326319800106 PM 24024698 ER PT J AU La Pierre, HS Minasian, SG Abubekerov, M Kozimor, SA Shuh, DK Tyliszczak, T Arnold, J Bergman, RG Toste, FD AF La Pierre, Henry S. Minasian, Stefan G. Abubekerov, Mark Kozimor, Stosh A. Shuh, David K. Tyliszczak, Tolek Arnold, John Bergman, Robert G. Toste, F. Dean TI Vanadium Bisimide Bonding Investigated by X-ray Crystallography, V-51 and C-13 Nuclear Magnetic Resonance Spectroscopy, and V L-3,L-2-Edge X-ray Absorption Near-Edge Structure Spectroscopy SO INORGANIC CHEMISTRY LA English DT Article ID C-H ACTIVATION; DENSITY-FUNCTIONAL THEORY; IMIDO COMPLEXES; ELECTRONIC-STRUCTURE; TRANSITION-METALS; ENANTIOSELECTIVE REDUCTION; ORGANOMETALLIC CHEMISTRY; ORGANOTITANIUM COMPLEXES; METALLOCENE DICHLORIDES; PROPYLENE AMMOXIDATION AB Syntheses of neutral halide and aryl vanadium bisimides are described. Treatment of VCl2(NtBu)[NTMS-((NBu)-Bu-t)], 2, with PMe3, PEt3, PMe2Ph, or pyridine gave vanadium bisimides via TMSC1 elimination in good yield: VCl(PMe3)(2)((NBu)-Bu-t)(2) 3, VCl(PEt3)(2)(NlBu)(2) 4, VCl(PMe2Ph)(2)((NBu)-Bu-t)(2) 5, and VCl(Py)(2)((NBu)-Bu-t)(2) 6. The halide series (Cl-I) was synthesized by use of TMSBr and TMSI to give VBr(PMe3)(2)((NBu)-Bu-t)(2) 7 and VI(PMe3)(2)((NBu)-Bu-t)(2) 8. The phenyl derivative was obtained by reaction of 3 with MgPh2 to give VPh(PMe3)(2)((NBu)-Bu-t)(2) 9. These neutral complexes are compared to the previously reported cationic bisimides [V(PMe3)(3)((NBu)-Bu-t)(2)][Al(PFTB)(4)] 10, [V(PEt3)(2)((NBu)-Bu-t)(2)][Al(PFTB)(4)] 11, and [V(DMAP)(PEt3)(2)((NBu)-Bu-t)(2)][Al(PFTB)(4)] 12 (DMAP = dimethylaminopyridine, PFTB = perfluoro-tert-butoxide). Characterization of the complexes by X-ray diffraction, C-13 NMR, V-51 NMR, and V L-3,L-2-edge X-ray absorption nearedge structure (XANES) spectroscopy provides a description of the electronic structure in comparison to group 6 bisimides and the bent metallocene analogues. The electronic structure is dominated by pi bonding to the imides, and localization of electron density at the nitrogen atoms of the imides is dictated by the cone angle and donating ability of the axial neutral supporting ligands. This phenomenon is clearly seen in the sensitivity of V-51 NMR shift, C-13 NMR Delta delta(alpha beta), and L-3-edge energy to the nature of the supporting phosphine ligand, which defines the parameters for designing cationic group 5 bisimides that would be capable of breaking stronger sigma bonds. Conversely, all three methods show little dependence on the variable equatorial halide ligand. Furthermore, this analysis allows for quantification of the electronic differences between vanadium bisimides and the structurally analogous mixed Cp/imide system CpV((NBu)-Bu-t)X-2 (Cp = C5H51-). C1 [La Pierre, Henry S.; Abubekerov, Mark; Arnold, John; Bergman, Robert G.; Toste, F. Dean] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Minasian, Stefan G.; Kozimor, Stosh A.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Minasian, Stefan G.; Shuh, David K.; Tyliszczak, Tolek] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Minasian, Stefan G.; Shuh, David K.; Tyliszczak, Tolek] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Arnold, J (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM arnold@berkeley.edu; rbergman@berkeley.edu; fdtoste@berkeley.edu RI Arnold, John/F-3963-2012; OI Arnold, John/0000-0001-9671-227X; Toste, F. Dean/0000-0001-8018-2198 FU NSF; UCB Department of Chemistry; AFOSR [11RSA093]; Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences (CSGB); U.S. Department of Energy at Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy at LBNL [DE-AC02-05CH11231]; Office of Science, Office of Basic Energy Sciences and by the Division of Chemical Sciences, Geosciences, and Biosciences, Heavy Element Chemistry program of the U.S. Department of Energy at LBNL [DE-AC02-05CH11231]; Heavy Element Chemistry Program at LANL by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy; National Nuclear Security Administration of U.S. Department of Energy [DE-AC52-06NA25396]; LANL by the Glenn T. Seaborg Institute postdoctoral fellowships FX H.S.LaP. acknowledges the support of NSF for a predoctoral fellowship and the UCB Department of Chemistry for the Dauben Fellowship. We thank Dr. Christopher Canlas for experimental assistance, and Professor Richard A. Andersen, Dr. Gregory Nocton, Dr. Neil C. Tomson, and Thomas L. Gianetti for helpful discussions. This work was supported at UC-Berkeley by the AFOSR (11RSA093). The MES Beamline 11.0.2 was supported by the Director, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences (CSGB) and the CSGB Condensed Phase and Interfacial Molecular Sciences program, both of the U.S. Department of Energy at Lawrence Berkeley National Laboratory under Contract No. DE-AC02-05CH11231. T.T. and the ALS were supported by Director, Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy at LBNL under Contract No. DE-AC02-05CH11231. D.K.S and S.G.M. (in part) were supported by Director, Office of Science, Office of Basic Energy Sciences and by the Division of Chemical Sciences, Geosciences, and Biosciences, Heavy Element Chemistry program of the U.S. Department of Energy at LBNL under Contract DE-AC02-05CH11231. S.A.K. was supported under the Heavy Element Chemistry Program at LANL by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy. Los Alamos National Laboratory is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of U.S. Department of Energy under Contract DE-AC52-06NA25396. Parts of this work were also supported at LANL by the Glenn T. Seaborg Institute postdoctoral fellowships (S.G.M.). NR 125 TC 6 Z9 6 U1 0 U2 34 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD OCT 7 PY 2013 VL 52 IS 19 BP 11650 EP 11660 DI 10.1021/ic4020543 PG 11 WC Chemistry, Inorganic & Nuclear SC Chemistry GA 243MF UT WOS:000326319800111 PM 24024833 ER PT J AU Baker, KL Stewart, RE Steele, PT Vernon, SP Hsing, WW Remington, BA AF Baker, K. L. Stewart, R. E. Steele, P. T. Vernon, S. P. Hsing, W. W. Remington, B. A. TI Solid-state framing camera with multiple time frames SO APPLIED PHYSICS LETTERS LA English DT Article ID FREE-ELECTRON LASERS; RAY; GAAS AB A high speed solid-state framing camera has been developed which can operate over a wide range of photon energies. This camera measures the two-dimensional spatial profile of the flux incident on a cadmium selenide semiconductor at multiple times. This multi-frame camera has been tested at 3.1 eV and 4.5 keV. The framing camera currently records two frames with a temporal separation between the frames of 5 ps but this separation can be varied between hundreds of femtoseconds up to nanoseconds and the number of frames can be increased by angularly multiplexing the probe beam onto the cadmium selenide semiconductor. (C) 2013 AIP Publishing LLC. C1 [Baker, K. L.; Stewart, R. E.; Steele, P. T.; Vernon, S. P.; Hsing, W. W.; Remington, B. A.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Baker, KL (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM Baker7@llnl.gov FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. The authors would like to acknowledge the JLF staff for their support of these experiments and in particular J. Bonlie, C. Filip, C. Cadwalader, R. Costa, G. Freeze, and S. Maricle. We also wish to acknowledge G. Loomis, P. Thelin, and J. Dela Fuente for optical coating, polishing, and manufacturing support. NR 23 TC 5 Z9 7 U1 0 U2 19 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD OCT 7 PY 2013 VL 103 IS 15 AR 151111 DI 10.1063/1.4824192 PG 4 WC Physics, Applied SC Physics GA 236FD UT WOS:000325779700011 ER PT J AU Chan, CWI Hu, Q Reno, JL AF Chan, Chun Wang I. Hu, Qing Reno, John L. TI Tall-barrier terahertz quantum cascade lasers SO APPLIED PHYSICS LETTERS LA English DT Article ID SEMICONDUCTORS AB A terahertz quantum cascade laser is presented in which selectively placed pure AlAs barriers are used to reduce parasitic leakage currents to the conduction band continuum. The design is demonstrated to have improved temperature performance over a regrowth of the current T-max similar to 200K record holder (181 K vs. 175 K). Strangely, it fails to lase below similar to 70 K, which we attribute to negative differential resistance (NDR) prior to threshold. A subsequent design using only AlAs barriers failed to lase, the reason for which we posit to be either early NDR or excessive interface roughness scattering. (C) 2013 AIP Publishing LLC. C1 [Chan, Chun Wang I.; Hu, Qing] MIT, Dept Elect Engn & Comp Sci, Cambridge, MA 02139 USA. [Reno, John L.] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA. RP Chan, CWI (reprint author), MIT, Dept Elect Engn & Comp Sci, Cambridge, MA 02139 USA. EM icwchan@mit.edu FU National Aeronautics and Space Administration; National Science Foundation; U.S. Department of Energy National Nuclear Security Administration [DE-AC04-94AL85000] FX The work at the Massachusetts Institute of Technology was supported by the National Aeronautics and Space Administration and the National Science Foundation. The work at Sandia was performed, in part, at the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences user facility. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 17 TC 8 Z9 8 U1 0 U2 22 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD OCT 7 PY 2013 VL 103 IS 15 AR 151117 DI 10.1063/1.4824878 PG 4 WC Physics, Applied SC Physics GA 236FD UT WOS:000325779700017 ER PT J AU Gan, ZF Perea, DE Yoo, J Picraux, ST Smith, DJ McCartney, MR AF Gan, Zhaofeng Perea, Daniel E. Yoo, Jinkyoung Picraux, S. Tom Smith, David J. McCartney, Martha R. TI Mapping electrostatic profiles across axial p-n junctions in Si nanowires using off-axis electron holography SO APPLIED PHYSICS LETTERS LA English DT Article ID DOPED SILICON NANOWIRES; GROWTH; ABRUPTNESS; RESOLUTION; ATOMS AB Si nanowires (NWs) with axial p-n junctions were grown by the vapor-liquid-solid method. Transmission electron microscopy and electron holography were used to characterize the microstructure and electrostatic properties. Measurement of the potential profile showed the presence of a p-n junction with a height of 1.0 +/- 0.3V. A Schottky barrier was observed at the end of the NW due to the Au catalyst particle. Comparison with simulations indicated dopant concentrations of 10(19) cm(-3) for donors and 10(17) cm(-3) for acceptors. These results confirm the benefit of combining off-axis electron holography with simulations for determining localized information about the electrically active dopant distributions in nanowire structures. (C) 2013 AIP Publishing LLC. C1 [Gan, Zhaofeng; Smith, David J.; McCartney, Martha R.] Arizona State Univ, Dept Phys, Tempe, AZ 85287 USA. [Perea, Daniel E.] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Yoo, Jinkyoung; Picraux, S. Tom] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. RP Gan, ZF (reprint author), Arizona State Univ, Dept Phys, Tempe, AZ 85287 USA. EM zgan2@asu.edu RI Yoo, Jinkyoung/B-5291-2008; Perea, Daniel/A-5345-2010 OI Yoo, Jinkyoung/0000-0002-9578-6979; FU DoE [DE-FG02-04ER46168]; Laboratory Directed Research and Development Program at LANL; National Nuclear Security Administration of the U.S. Department of Energy [DE-AC52-06NA25396]; Department of Energy's Office of Biological and Environmental Research FX The electron holography studies have been supported by DoE Grant No. DE-FG02-04ER46168. This work was performed in part at CINT, a U.S. Department of Energy, Office of Science User Facility. The research was funded in part by the Laboratory Directed Research and Development Program at LANL, an affirmative action equal opportunity employer operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy under Contract No. DE-AC52-06NA25396. A portion of the research was also performed using EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. We gratefully acknowledge the use of facilities within the John M. Cowley Center for High Resolution Electron Microscopy at Arizona State University, and we also thank Professor Karen Kavanagh at Simon Fraser University for microscope access and Professor Dragica Vasileska for helpful discussions. NR 24 TC 8 Z9 8 U1 2 U2 37 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD OCT 7 PY 2013 VL 103 IS 15 AR 153108 DI 10.1063/1.4824775 PG 5 WC Physics, Applied SC Physics GA 236FD UT WOS:000325779700069 ER PT J AU Shi, TT Yin, WJ Al-Jassim, M Yan, YF AF Shi, Tingting Yin, Wan-Jian Al-Jassim, Mowafak Yan, Yanfa TI Structural, electronic, and optical properties of Cu-3-V-VI4 compound semiconductors SO APPLIED PHYSICS LETTERS LA English DT Article ID NORMAL TETRAHEDRAL STRUCTURES; TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; FILM SOLAR-CELLS; CRYSTAL-STRUCTURE; BASIS-SET; REFINEMENT; EFFICIENCY; CUINSE2; ENARGITE AB Cu-V-VII chalcogenide semiconductors have recently been considered promising earth-abundant solar cell materials. Using first-principles density-functional theory with hybrid functional, we have studied the structural, electronic, and optical properties of Cu-3-V-VI4 compounds. We find that Cu3PS4 and Cu3PSe4 prefer energetically the enargite structure, whereas other compounds favor the famatinite structure. The Cu-3-V-VI4 family exhibits bandgaps ranging from 0.88 eV to 2.51 eV, revealing the potentials for both single junction and multijunction solar cell applications. The calculated bandgaps for Cu-3-V-VI4 compounds are in good agreement with the available theoretical and experimental results. (C) 2013 AIP Publishing LLC. C1 [Shi, Tingting; Yin, Wan-Jian; Yan, Yanfa] Univ Toledo, Dept Phys & Astron, Toledo, OH 43606 USA. [Shi, Tingting; Yin, Wan-Jian; Yan, Yanfa] Univ Toledo, Wright Ctr Photovolta Innovat & Commercializat, Toledo, OH 43606 USA. [Al-Jassim, Mowafak] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Yan, YF (reprint author), Univ Toledo, Dept Phys & Astron, 2801 Bancroft St, Toledo, OH 43606 USA. EM yanfa.yan@utoledo.edu RI Yin, Wanjian/F-6738-2013 FU Ohio Research Scholar Program (ORSP); U.S. Department of Energy [DE-AC36-08GO28308]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX Y.Y. acknowledges the support from the Ohio Research Scholar Program (ORSP). Work at NREL was supported by the U.S. Department of Energy under Contract No. DE-AC36-08GO28308. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 34 TC 6 Z9 6 U1 1 U2 46 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD OCT 7 PY 2013 VL 103 IS 15 AR 152105 DI 10.1063/1.4824770 PG 4 WC Physics, Applied SC Physics GA 236FD UT WOS:000325779700043 ER PT J AU Kim, KH Kim, E Kim, H Tappero, R Bolotnikov, AE Camarda, GS Hossain, A Cirignano, L James, RB AF Kim, Ki Hyun Kim, Eunlim Kim, H. Tappero, R. Bolotnikov, A. E. Camarda, G. S. Hossain, A. Cirignano, L. James, R. B. TI Electro-migration of impurities in TlBr SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID DETECTORS; DEGRADATION; CRYSTALS; ELECTROMIGRATION; SEMICONDUCTORS; CONDUCTIVITY AB We observed the electro-migration of Cu, Ag, and Au impurities that exist in positive-ion states in TlBr detectors under electric field strengths typically used for device operation. The migration occurred predominantly through bulk-and specific-channels, which are presumed to be a network of grain and sub-grain boundaries. The electro-migration velocity of Cu, Ag, and Au in TlBr is about 4-8 x 10(-8) cm/s at room temperature under an electric field of 500-800 V/mm. The instability and polarization effects of TlBr detectors might well be correlated with the electro-migration of residual impurities in TlBr, which alters the internal electric field over time. The effect may also have been due to migration of the electrode material itself, which would allow for the possibility of a better choice for contact material and for depositing an effective diffusion barrier. From our findings, we suggest that applying our electro-migration technique for purifying material is a promising new way to remove electrically active metallic impurities in TlBr crystals, as well as other materials. (C) 2013 AIP Publishing LLC. C1 [Kim, Ki Hyun; Kim, Eunlim] Korea Univ, Dept Radiol Sci, Seoul 136703, South Korea. [Kim, H.; Cirignano, L.] Radiat Monitoring Devices Inc, Watertown, MA 02472 USA. [Tappero, R.; Bolotnikov, A. E.; Camarda, G. S.; Hossain, A.; James, R. B.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Kim, KH (reprint author), Korea Univ, Dept Radiol Sci, Seoul 136703, South Korea. EM khkim1@korea.ac.kr FU Korea University [K1222241]; U.S. Department of Energy, Office of Nonproliferation Research and Verification [NA-22] FX This work was supported by Korea University (K1222241) and the U.S. Department of Energy, Office of Nonproliferation Research and Verification, NA-22. NR 18 TC 1 Z9 1 U1 2 U2 13 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD OCT 7 PY 2013 VL 114 IS 13 AR 133701 DI 10.1063/1.4823781 PG 6 WC Physics, Applied SC Physics GA 232JB UT WOS:000325488700018 ER PT J AU Newman, BK Ertekin, E Sullivan, JT Winkler, MT Marcus, MA Fakra, SC Sher, MJ Mazur, E Grossman, JC Buonassisi, T AF Newman, Bonna K. Ertekin, Elif Sullivan, Joseph T. Winkler, Mark T. Marcus, Matthew A. Fakra, Sirine C. Sher, Meng-Ju Mazur, Eric Grossman, Jeffrey C. Buonassisi, Tonio TI Extended X-ray absorption fine structure spectroscopy of selenium-hyperdoped silicon SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID LASER-MICROSTRUCTURED SILICON; INFRARED-ABSORPTION; DOPED SILICON; FEMTOSECOND; SULFUR; NUMBER; IRRADIATION; SPECIATION; IFEFFIT; ORDER AB Silicon doped with an atomic percent of chalcogens exhibits strong, uniform sub-bandgap optical absorptance and is of interest for photovoltaic and infrared detector applications. This sub-bandgap absorptance is reduced with subsequent thermal annealing indicative of a diffusion mediated chemical change. However, the precise atomistic origin of absorptance and its deactivation is unclear. Herein, we apply Se K-edge extended X-ray absorption fine structure (EXAFS) spectroscopy to probe the chemical states of selenium dopants in selenium-hyperdoped silicon annealed to varying degrees. We observe a smooth and continuous selenium chemical state change with increased annealing temperature, highly correlated to the decrease in sub-bandgap optical absorptance. In samples exhibiting strong sub-bandgap absorptance, EXAFS analysis reveals that the atoms nearest to the Se atom are Si at distances consistent with length scales in energetically favorable Se substitutional-type point defect complexes as calculated by density functional theory. As the sub-bandgap absorptance increases, EXAFS data indicate an increase in the Se-Si bond distance. In specimens annealed at 1225 K exhibiting minimal sub-bandgap absorptance, fitting of the EXAFS spectra indicates that Se is predominantly in a silicon diselenide (SiSe2) precipitate state. The EXAFS study supports a model of highly optically absorbing point defects that precipitate during annealing into structures with no sub-bandgap absorptance. (C) 2013 AIP Publishing LLC. C1 [Newman, Bonna K.; Ertekin, Elif; Sullivan, Joseph T.; Winkler, Mark T.; Grossman, Jeffrey C.; Buonassisi, Tonio] MIT, Cambridge, MA 02139 USA. [Marcus, Matthew A.; Fakra, Sirine C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Sher, Meng-Ju; Mazur, Eric] Harvard Univ, Cambridge, MA 02138 USA. RP Newman, BK (reprint author), FOM Inst AMOLF, NL-1098 XG Amsterdam, Netherlands. EM bonna@alum.mit.edu; ertekin@illinois.edu; buonassisi@mit.edu RI Ertekin, Elif/D-6764-2013 FU Chesonis Family Foundation; National Science Foundation (NSF); Department of Energy (DOE) under NSF CA [EEC-1041895, CBET 0754227, CHE-DMR-DNS 0934480]; Claire Boothe Luce Family Foundation; Office of Science, Office of Basic Energy Sciences, US Department of Energy [DE-AC02-05CH11231]; NSF [ECS-0335765] FX We gratefully acknowledge Bruce Ravel for assistance with fitting of the EXAFS data. This research was supported by the Chesonis Family Foundation, the National Science Foundation (NSF), and the Department of Energy (DOE) under NSF CA Nos. EEC-1041895, and CBET 0754227, and CHE-DMR-DNS 0934480. B. K. N. acknowledges support from the Claire Boothe Luce Family Foundation. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, US Department of Energy under Contract No. DE-AC02-05CH11231. We also acknowledge the Center for Nanoscale Systems at Harvard University, which is a member of the National Nanotechnology Infrastructure Network (NNIN) that is supported by the NSF under Award No. ECS-0335765. NR 42 TC 11 Z9 11 U1 2 U2 31 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD OCT 7 PY 2013 VL 114 IS 13 AR 133507 DI 10.1063/1.4824279 PG 8 WC Physics, Applied SC Physics GA 232JB UT WOS:000325488700014 ER PT J AU Smith, RF Bolme, CA Erskine, DJ Celliers, PM Ali, S Eggert, JH Brygoo, SL Hammel, BD Wang, J Collins, GW AF Smith, R. F. Bolme, C. A. Erskine, D. J. Celliers, P. M. Ali, S. Eggert, J. H. Brygoo, S. L. Hammel, B. D. Wang, J. Collins, G. W. TI Heterogeneous flow and brittle failure in shock-compressed silicon SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID PHASE-TRANSITION; INTERFEROMETER; WAVE; PRESSURE; STRENGTH; FRACTURE; BISMUTH; MODULI AB We combine a recently developed high-resolution two-dimensional (2D) imaging velocimetry technique (velocity interferometer system for any reflector (VISAR)) with 1D VISAR measurements to construct a moving picture of heterogeneous deformation in shock-compressed single crystal silicon. The 2D VISAR takes an intensity snapshot of target velocity and reflectivity over a mm field-of-view while the compression history is simultaneously recorded by the 1D VISAR. Our data show particle velocity surface roughening due to the anisotropic onset of plasticity and, above similar to 13 GPa, a structural phase transformation. Shock arrival at the Si free-surface is characterized by the formation of fracture networks and incipient velocity jetting. (C) 2013 AIP Publishing LLC. C1 [Smith, R. F.; Erskine, D. J.; Celliers, P. M.; Ali, S.; Eggert, J. H.; Hammel, B. D.; Collins, G. W.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Bolme, C. A.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Ali, S.] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. [Brygoo, S. L.] CEA, DAM, DIF, F-91297 Arpajon, France. [Wang, J.] Princeton Univ, Dept Geosci, Princeton, NJ 08544 USA. RP Smith, RF (reprint author), Lawrence Livermore Natl Lab, POB 808, Livermore, CA 94551 USA. RI Wang, Jue/I-4705-2014; OI Wang, Jue/0000-0001-9206-4367; Bolme, Cynthia/0000-0002-1880-271X FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; National Laser User's Facility Award [DE-NA0000856] FX We thank Stephanie Uhlich and Walter Unites for help in the target preparation, Jim Cox for the engineering support in construction of the 2D VISAR, and the staff at the Jupiter Laser Facility at LLNL. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. J.W.'s participation was supported by National Laser User's Facility Award No. DE-NA0000856. NR 33 TC 6 Z9 6 U1 2 U2 39 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD OCT 7 PY 2013 VL 114 IS 13 AR 133504 DI 10.1063/1.4820927 PG 11 WC Physics, Applied SC Physics GA 232JB UT WOS:000325488700011 ER PT J AU Yang, XD Hu, CY Deng, HX Rosenmann, D Czaplewski, DA Gao, J AF Yang, Xiaodong Hu, Changyu Deng, Huixu Rosenmann, Daniel Czaplewski, David A. Gao, Jie TI Experimental demonstration of near-infrared epsilon-near-zero multilayer metamaterial slabs SO OPTICS EXPRESS LA English DT Article ID COMPLEX REFRACTIVE-INDEX; NEGATIVE REFRACTION; TRANSMITTANCE; TRANSITIONS; REFLECTANCE; LIGHT AB Near-infrared epsilon-near-zero (ENZ) metamaterial slabs based on silver-germanium (Ag-Ge) multilayers are experimentally demonstrated. Transmission, reflection and absorption spectra are characterized and used to determine the complex refractive indices and the effective permittivities of the ENZ metamaterial slabs, which match the results obtained from both the numerical simulations and the optical nonlocalities analysis. A rapid post-annealing process is used to reduce the collision frequency of silver and therefore decrease the optical absorption loss of multilayer metamaterial slabs. Furthermore, multilayer grating structures are studied to enhance the optical transmission and also tune the location of ENZ wavelength. The demonstrated near-infrared ENZ multilayer metamaterial slabs are important for realizing many exotic applications, such as phase front shaping and engineering of photonic density of states. (C) 2013 Optical Society of America C1 [Yang, Xiaodong; Hu, Changyu; Deng, Huixu; Gao, Jie] Missouri Univ Sci & Technol, Dept Mech & Aerosp Engn, Rolla, MO 65409 USA. [Rosenmann, Daniel; Czaplewski, David A.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. RP Yang, XD (reprint author), Missouri Univ Sci & Technol, Dept Mech & Aerosp Engn, Rolla, MO 65409 USA. EM yangxia@mst.edu; gaojie@mst.edu FU Intelligent Systems Center at Missouri ST; Energy Research and Development Center at Missouri ST; Materials Research Center at Missouri ST; University of Missouri Research Board; U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work was partially supported by the Intelligent Systems Center, the Energy Research and Development Center and the Materials Research Center at Missouri S&T, and the University of Missouri Research Board. The use of the Center for Nanoscale Materials was supported by the U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. The authors acknowledge L. Sun for his useful discussions about this work. NR 41 TC 11 Z9 11 U1 1 U2 44 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD OCT 7 PY 2013 VL 21 IS 20 BP 23631 EP 23639 DI 10.1364/OE.21.023631 PG 9 WC Optics SC Optics GA 233EU UT WOS:000325549800060 PM 24104275 ER PT J AU Feng, YJ Silevitch, DM Wang, JY Palmer, A Woo, N Yan, JQ Islam, Z Suslov, AV Littlewood, PB Rosenbaum, TF AF Feng, Yejun Silevitch, D. M. Wang, Jiyang Palmer, A. Woo, Nayoon Yan, J. -Q. Islam, Z. Suslov, A. V. Littlewood, P. B. Rosenbaum, T. F. TI Evolution of incommensurate spin order with magnetic field and temperature in the itinerant antiferromagnet GdSi SO PHYSICAL REVIEW B LA English DT Article ID X-RAY-SCATTERING; NEUTRON-DIFFRACTION; CHROMIUM; CRYSTAL; RNI2GE2; R=GD; TM AB GdSi exhibits spin-density-wave (SDW) order arising from the cooperative interplay of sizeable local moments and a partially nested Fermi sea of itinerant electrons. Using magnetotransport, magnetization, and nonresonant magnetic x-ray diffraction techniques, we determine the H-T phase diagrams of GdSi for magnetic fields up to 21 T, where antiferromagnetic order is no longer stable, and field directions along each of the three major crystal axes. While the incommensurate magnetic ordering vector that characterizes the SDW is robust under magnetic field, the multiple spin structures of this compound are highly flexible and rotate relative to the applied field via either canting or spin-flop processes. The antiferromagnetic spin densities always arrange themselves transverse to the applied magnetic field direction. The phase diagrams are delineated by two types of phase boundaries: one separates a collinear from a planar spin structure associated with a lattice structural transition, and the other defines a spin flop transition that is only weakly temperature dependent. The major features of the phase diagrams along each of the crystal axes can be explained by the combination of local moment and global Fermi surface physics at play. C1 [Feng, Yejun; Islam, Z.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Feng, Yejun; Silevitch, D. M.; Wang, Jiyang; Palmer, A.; Woo, Nayoon; Littlewood, P. B.; Rosenbaum, T. F.] Univ Chicago, James Franck Inst, Chicago, IL 60637 USA. [Feng, Yejun; Silevitch, D. M.; Wang, Jiyang; Palmer, A.; Woo, Nayoon; Littlewood, P. B.; Rosenbaum, T. F.] Univ Chicago, Dept Phys, Chicago, IL 60637 USA. [Yan, J. -Q.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Yan, J. -Q.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Suslov, A. V.] Natl High Magnet Field Lab, Tallahassee, FL 32310 USA. [Littlewood, P. B.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Feng, YJ (reprint author), Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RI Suslov, Alexey/M-7511-2014; Feng, Yejun/A-5417-2009 OI Suslov, Alexey/0000-0002-2224-153X; Feng, Yejun/0000-0003-3667-056X FU National Science Foundation [1206519]; NSF [DMR-0820054]; U.S. Department of Energy Basic Energy Sciences [NE-AC02-06CH11357]; National Science Foundation Cooperative Agreement [DMR-1157490]; State of Florida; U.S. Department of Energy; Materials Sciences and Engineering Division, DOE-BES; DOE-SCGF [DE-AC05-06OR23100] FX The work at the University of Chicago was supported by National Science Foundation Grant No. 1206519 and used MRSEC shared facilities, NSF Grant No. DMR-0820054. The work at the Advanced Photon Source of Argonne National Laboratory was supported by the U.S. Department of Energy Basic Energy Sciences under Contract No. NE-AC02-06CH11357. Work performed at the National High Magnetic Field Laboratory was supported by National Science Foundation Cooperative Agreement No. DMR-1157490, the State of Florida, and the U.S. Department of Energy. Work at Oak Ridge National Laboratory was supported by the Materials Sciences and Engineering Division, DOE-BES. A. P. was supported in part by DOE-SCGF under Contract DE-AC05-06OR23100. NR 30 TC 1 Z9 1 U1 1 U2 24 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 7 PY 2013 VL 88 IS 13 AR 134404 DI 10.1103/PhysRevB.88.134404 PG 8 WC Physics, Condensed Matter SC Physics GA 232LX UT WOS:000325496400002 ER PT J AU Manes, JL de Juan, F Sturla, M Vozmediano, MAH AF Manes, Juan L. de Juan, Fernando Sturla, Mauricio Vozmediano, Maria A. H. TI Generalized effective Hamiltonian for graphene under nonuniform strain SO PHYSICAL REVIEW B LA English DT Article ID ELECTRONIC-PROPERTIES; DIRAC FERMIONS; BAND-STRUCTURE; SHEETS AB We use a symmetry approach to construct a systematic derivative expansion of the low-energy effective Hamiltonian modifying the continuum Dirac description of graphene in the presence of nonuniform elastic deformations. We extract all experimentally relevant terms and describe their physical significance. Among them there is a new gap-opening term that describes the Zeeman coupling of the elastic pseudomagnetic field and the pseudospin. We determine the value of the couplings using a generalized tight-binding model. C1 [Manes, Juan L.] Univ Basque Country, Dept Fis Mat Condensada, E-48080 Bilbao, Spain. [de Juan, Fernando] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [de Juan, Fernando] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Sturla, Mauricio; Vozmediano, Maria A. H.] Inst Ciencia Mat, Madrid 28049, Spain. [Sturla, Mauricio; Vozmediano, Maria A. H.] CSIC, E-28049 Madrid, Spain. RP Manes, JL (reprint author), Univ Basque Country, Dept Fis Mat Condensada, Apartado 644, E-48080 Bilbao, Spain. RI de Juan, Fernando/B-9392-2008; Vozmediano, Maria/A-1391-2009 OI de Juan, Fernando/0000-0001-6852-1484; Vozmediano, Maria/0000-0003-2574-2310 FU Spanish MECD [FIS2011-23713, PIB2010BZ-00512, FPA2009-10612, FPA2012-34456]; Spanish Consolider-Ingenio Programme CPAN [CSD2007-00042]; Basque Government [IT559-10]; NSF [DRM-1005035]; "Programa Nacional de Movilidad de Recursos Humanos" (Spanish MECD) FX We thank A. Cortijo, A. G. Grushin, H. Ochoa, and E. da Silva for useful conversations. This research was supported by Spanish MECD Grants No. FIS2011-23713, No. PIB2010BZ-00512, No. FPA2009-10612, and No. FPA2012-34456, the Spanish Consolider-Ingenio 2010 Programme CPAN (Grant No. CSD2007-00042), by Basque Government Grant No. IT559-10 and by NSF Grant No. DRM-1005035. F.d.J. acknowledges funding from the "Programa Nacional de Movilidad de Recursos Humanos" (Spanish MECD). NR 65 TC 34 Z9 34 U1 4 U2 32 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 7 PY 2013 VL 88 IS 15 AR 155405 DI 10.1103/PhysRevB.88.155405 PG 10 WC Physics, Condensed Matter SC Physics GA 232NL UT WOS:000325500600006 ER PT J AU Yan, JQ Saparov, B Sefat, AS Yang, H Cao, HB Zhou, HD Sales, BC Mandrus, DG AF Yan, J. -Q. Saparov, B. Sefat, A. S. Yang, H. Cao, H. B. Zhou, H. D. Sales, B. C. Mandrus, D. G. TI Absence of structural transition in M0.5IrTe2 (M = Mn, Fe, Co, Ni) SO PHYSICAL REVIEW B LA English DT Article ID BAND-STRUCTURE; IRTE2; RESISTANCE; CUIR2TE4; CRYSTAL; FETE2; COTE2 AB M-doped IrTe2 (M=Mn, Fe, Co, Ni) compounds were synthesized by solid-state reaction. Single crystal x-ray diffraction experiments indicate that part of the doped M ions (M= Fe, Co, and Ni) substitute for Ir, and the rest intercalate into the octahedral interstitial sites located in between IrTe2 layers. Due to the lattice mismatch between MnTe2 and IrTe2, Mn has limited solubility in IrTe2 lattice. The trigonal structure is stable in the whole temperature range 1.80 K <= T <= 300 K for all doped compositions. No long-range magnetic order or superconductivity was observed in any doped compositions above 1.80 K. A spin glass behavior below 10 K was observed in Fe-doped IrTe2 from the temperature dependence of magnetization, electrical resistivity, and specific heat. The low temperature specific heat data suggest the electron density of states is enhanced in Fe-and Co-doped compositions but reduced in Ni-doped IrTe2. With the 3d transition metal doping the trigonal a-lattice parameter increases but the c-lattice parameter decreases. Detailed analysis of the single crystal x-ray diffraction data shows that interlayer Te-Te distance increases despite a reduced c lattice. The importance of the Te-Te, Te-Ir, and Ir-Ir bonding is discussed. C1 [Yan, J. -Q.; Saparov, B.; Sefat, A. S.; Sales, B. C.; Mandrus, D. G.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Yan, J. -Q.; Yang, H.; Mandrus, D. G.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Yang, H.] Northeastern Univ, Inst Mat & Met, Shenyang 110004, Peoples R China. [Cao, H. B.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Zhou, H. D.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. RP Yan, JQ (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RI Mandrus, David/H-3090-2014; Cao, Huibo/A-6835-2016; Zhou, Haidong/O-4373-2016; Sefat, Athena/R-5457-2016 OI Cao, Huibo/0000-0002-5970-4980; Sefat, Athena/0000-0002-5596-3504 FU US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division FX J.Q.Y. thanks Minghu Pan for helpful discussions. B. I. S. and H. B. C. thank R. Custelcean for his assistance with the single crystal x-ray diffraction measurements. Work at ORNL was supported by the US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. NR 23 TC 3 Z9 3 U1 12 U2 60 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 EI 1550-235X J9 PHYS REV B JI Phys. Rev. B PD OCT 7 PY 2013 VL 88 IS 13 AR 134502 DI 10.1103/PhysRevB.88.134502 PG 7 WC Physics, Condensed Matter SC Physics GA 232LX UT WOS:000325496400005 ER PT J AU Moriya, K Schumacher, RA Adhikari, KP Adikaram, D Aghasyan, M Amaryan, MJ Anderson, MD Pereira, SA Avakian, H Ball, J Baltzell, NA Battaglieri, M Batourine, V Bedlinskiy, I Bellis, M Bennett, RP Biselli, AS Bono, J Boiarinov, S Briscoe, WJ Brooks, WK Burkert, VD Carman, DS Celentano, A Chandavar, S Collins, P Contalbrigo, M Cortes, O Crede, V D'Angelo, A Dashyan, N De Vita, R De Sanctis, E Deur, A Dey, B Djalali, C Doughty, D Dugger, M Dupre, R Egiyan, H El Fassi, L Eugenio, P Fedotov, G Fegan, S Fersch, R Fleming, JA Gevorgyan, N Gilfoyle, GP Giovanetti, KL Girod, FX Goetz, JT Gohn, W Golovatch, E Gothe, RW Griffioen, KA Guidal, M Guler, N Guo, L Hakobyan, H Hanretty, C Heddle, D Hicks, K Ho, D Holtrop, M Ilieva, Y Ireland, DG Ishkhanov, BS Isupov, EL Jo, HS Joo, K Keller, D Khandaker, M Klein, A Klein, FJ Koirala, S Kubarovsky, A Kubarovsky, V Kuleshov, SV Lewis, S Livingston, K Lu, HY MacGregor, IJD Martinez, D Mayer, M McCracken, M McKinnon, B Mestayer, MD Meyer, CA Mineeva, T Mirazita, M Mokeev, V Montgomery, RA Moutarde, H Munevar, E Camacho, CM Nadel-Turonski, P Nasseripour, R Nepali, CS Niccolai, S Niculescu, G Niculescu, I Osipenko, M Ostrovidov, AI Pappalardo, LL Paremuzyan, R Park, K Park, S Pasyuk, E Phelps, E Phillips, JJ Pisano, S Pogorelko, O Pozdniakov, S Price, JW Procureur, S Protopopescu, D Puckett, AJR Raue, BA Rimal, D Ripani, M Ritchie, BG Rosner, G Rossi, P Sabatie, F Saini, MS Salgado, C Schott, D Seder, E Seraydaryan, H Sharabian, YG Smith, GD Sober, DI Sokhan, D Stepanyan, S Stoler, P Strauch, S Taiuti, M Tang, W Taylor, CE Taylor, S Tian, Y Tkachenko, S Ungaro, M Vernarsky, B Vineyard, MF Voskanyan, H Voutier, E Walford, NK Watts, DP Weinstein, LB Williams, M Wood, MH Zachariou, N Zana, L Zhang, J Zhao, ZW Zonta, I AF Moriya, K. Schumacher, R. A. Adhikari, K. P. Adikaram, D. Aghasyan, M. Amaryan, M. J. Anderson, M. D. Pereira, S. Anefalos Avakian, H. Ball, J. Baltzell, N. A. Battaglieri, M. Batourine, V. Bedlinskiy, I. Bellis, M. Bennett, R. P. Biselli, A. S. Bono, J. Boiarinov, S. Briscoe, W. J. Brooks, W. K. Burkert, V. D. Carman, D. S. Celentano, A. Chandavar, S. Collins, P. Contalbrigo, M. Cortes, O. Crede, V. D'Angelo, A. Dashyan, N. De Vita, R. De Sanctis, E. Deur, A. Dey, B. Djalali, C. Doughty, D. Dugger, M. Dupre, R. Egiyan, H. El Fassi, L. Eugenio, P. Fedotov, G. Fegan, S. Fersch, R. Fleming, J. A. Gevorgyan, N. Gilfoyle, G. P. Giovanetti, K. L. Girod, F. X. Goetz, J. T. Gohn, W. Golovatch, E. Gothe, R. W. Griffioen, K. A. Guidal, M. Guler, N. Guo, L. Hakobyan, H. Hanretty, C. Heddle, D. Hicks, K. Ho, D. Holtrop, M. Ilieva, Y. Ireland, D. G. Ishkhanov, B. S. Isupov, E. L. Jo, H. S. Joo, K. Keller, D. Khandaker, M. Klein, A. Klein, F. J. Koirala, S. Kubarovsky, A. Kubarovsky, V. Kuleshov, S. V. Lewis, S. Livingston, K. Lu, H. Y. MacGregor, I. J. D. Martinez, D. Mayer, M. McCracken, M. McKinnon, B. Mestayer, M. D. Meyer, C. A. Mineeva, T. Mirazita, M. Mokeev, V. Montgomery, R. A. Moutarde, H. Munevar, E. Camacho, C. Munoz Nadel-Turonski, P. Nasseripour, R. Nepali, C. S. Niccolai, S. Niculescu, G. Niculescu, I. Osipenko, M. Ostrovidov, A. I. Pappalardo, L. L. Paremuzyan, R. Park, K. Park, S. Pasyuk, E. Phelps, E. Phillips, J. J. Pisano, S. Pogorelko, O. Pozdniakov, S. Price, J. W. Procureur, S. Protopopescu, D. Puckett, A. J. R. Raue, B. A. Rimal, D. Ripani, M. Ritchie, B. G. Rosner, G. Rossi, P. Sabatie, F. Saini, M. S. Salgado, C. Schott, D. Seder, E. Seraydaryan, H. Sharabian, Y. G. Smith, G. D. Sober, D. I. Sokhan, D. Stepanyan, S. Stoler, P. Strauch, S. Taiuti, M. Tang, W. Taylor, C. E. Taylor, S. Tian, Y. Tkachenko, S. Ungaro, M. Vernarsky, B. Vineyard, M. F. Voskanyan, H. Voutier, E. Walford, N. K. Watts, D. P. Weinstein, L. B. Williams, M. Wood, M. H. Zachariou, N. Zana, L. Zhang, J. Zhao, Z. W. Zonta, I. CA CLAS Collaboration TI Differential photoproduction cross sections of the Sigma(0)(1385), Lambda(1405), and Lambda(1520) SO PHYSICAL REVIEW C LA English DT Article ID SCATTERING; HYPERON; STATES; MASSES AB We report the exclusive photoproduction cross sections for the Sigma(0)(1385), Lambda(1405), and Lambda(1520) in the reactions gamma + p -> K+ + Y* using the CLAS detector for energies from near the respective production thresholds up to a center-of-mass energy W of 2.85 GeV. The differential cross sections are integrated to give the total exclusive cross sections for each hyperon. Comparisons are made to current theoretical models based on the effective-Lagrangian approach and fit to previous data. The accuracy of these models is seen to vary widely. The cross sections for the Lambda(1405) region are strikingly different for the Sigma(+)pi(-), Sigma(0)pi(0), and Sigma(-)pi(+) decay channels, indicating the effect of isospin interference, especially at W values close to the threshold. C1 [Moriya, K.; Schumacher, R. A.; Bellis, M.; Biselli, A. S.; Dey, B.; Ho, D.; Lu, H. Y.; McCracken, M.; Meyer, C. A.; Vernarsky, B.; Williams, M.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Baltzell, N. A.; El Fassi, L.] Argonne Natl Lab, Argonne, IL 60439 USA. [Dugger, M.; Pasyuk, E.; Ritchie, B. G.] Arizona State Univ, Tempe, AZ 85287 USA. [Price, J. W.] Calif State Univ Dominguez Hills, Carson, CA 90747 USA. [Wood, M. H.] Canisius Coll, Buffalo, NY 14208 USA. [Collins, P.; Klein, F. J.; Sober, D. I.; Walford, N. K.] Catholic Univ Amer, Washington, DC 20064 USA. [Ball, J.; Girod, F. X.; Moutarde, H.; Procureur, S.; Sabatie, F.] CEA, Ctr Saclay, Irfu Serv Phys Nucl, F-91191 Gif Sur Yvette, France. [Doughty, D.; Fersch, R.; Heddle, D.] Christopher Newport Univ, Newport News, VA 23606 USA. [Gohn, W.; Joo, K.; Kubarovsky, A.; Mineeva, T.; Seder, E.; Ungaro, M.] Univ Connecticut, Storrs, CT 06269 USA. [Fleming, J. A.; Watts, D. P.] Univ Edinburgh, Edinburgh EH9 3JZ, Midlothian, Scotland. [Biselli, A. S.] Fairfield Univ, Fairfield, CT 06824 USA. [Bono, J.; Guo, L.; Raue, B. A.; Rimal, D.] Florida Int Univ, Miami, FL 33199 USA. [Crede, V.; Eugenio, P.; Hanretty, C.; Ostrovidov, A. I.; Park, S.; Saini, M. S.] Florida State Univ, Tallahassee, FL 32306 USA. [Taiuti, M.] Univ Genoa, I-16146 Genoa, Italy. [Briscoe, W. J.; Ilieva, Y.; Munevar, E.; Schott, D.; Strauch, S.] George Washington Univ, Washington, DC 20052 USA. [Cortes, O.; Martinez, D.; Taylor, C. E.] Idaho State Univ, Pocatello, ID 83209 USA. [Contalbrigo, M.; Pappalardo, L. L.] Ist Nazl Fis Nucl, Sez Ferrara, I-44100 Ferrara, Italy. [Aghasyan, M.; Pereira, S. Anefalos; De Sanctis, E.; Mirazita, M.; Pisano, S.; Rossi, P.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Battaglieri, M.; Celentano, A.; De Vita, R.; Fegan, S.; Osipenko, M.; Ripani, M.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [D'Angelo, A.; Zonta, I.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, I-00133 Rome, Italy. [Dupre, R.; Guidal, M.; Jo, H. S.; Camacho, C. Munoz; Niccolai, S.; Paremuzyan, R.] Inst Phys Nucl, F-91406 Orsay, France. [Bedlinskiy, I.; Kuleshov, S. V.; Pogorelko, O.; Pozdniakov, S.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Giovanetti, K. L.; Nasseripour, R.; Niculescu, G.; Niculescu, I.] James Madison Univ, Harrisonburg, VA 22807 USA. [Batourine, V.; Park, K.] Kyungpook Natl Univ, Taegu 702701, South Korea. [Voutier, E.] Univ Grenoble 1, CNRS, IN2P3, LPSC,INPG, Grenoble, France. [Holtrop, M.; Zana, L.] Univ New Hampshire, Durham, NH 03824 USA. [Khandaker, M.; Salgado, C.] Norfolk State Univ, Norfolk, VA 23504 USA. [Chandavar, S.; Goetz, J. T.; Hicks, K.; Tang, W.] Ohio Univ, Athens, OH 45701 USA. [Adhikari, K. P.; Adikaram, D.; Amaryan, M. J.; Bennett, R. P.; Guler, N.; Klein, A.; Koirala, S.; Mayer, M.; Nepali, C. S.; Seraydaryan, H.; Weinstein, L. B.] Old Dominion Univ, Norfolk, VA 23529 USA. [Kubarovsky, V.; Stoler, P.; Ungaro, M.] Rensselaer Polytech Inst, Troy, NY 12180 USA. [Gilfoyle, G. P.] Univ Richmond, Richmond, VA 23173 USA. [D'Angelo, A.] Univ Roma Tor Vergata, I-00133 Rome, Italy. [Fedotov, G.; Golovatch, E.; Ishkhanov, B. S.; Isupov, E. L.; Kubarovsky, A.; Mokeev, V.] Skobeltsyn Nucl Phys Inst, Moscow 119899, Russia. [Baltzell, N. A.; Djalali, C.; Fedotov, G.; Gothe, R. W.; Ilieva, Y.; Lu, H. Y.; Nasseripour, R.; Phelps, E.; Strauch, S.; Tian, Y.; Wood, M. H.; Zachariou, N.] Univ S Carolina, Columbia, SC 29208 USA. [Avakian, H.; Batourine, V.; Boiarinov, S.; Brooks, W. K.; Burkert, V. D.; Carman, D. S.; Deur, A.; Doughty, D.; Egiyan, H.; Girod, F. X.; Guo, L.; Heddle, D.; Kubarovsky, V.; Mestayer, M. D.; Mokeev, V.; Munevar, E.; Nadel-Turonski, P.; Park, K.; Pasyuk, E.; Puckett, A. J. R.; Raue, B. A.; Sharabian, Y. G.; Stepanyan, S.; Taylor, S.; Ungaro, M.; Zhang, J.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. [Vineyard, M. F.] Union Coll, Schenectady, NY 12308 USA. [Brooks, W. K.; Hakobyan, H.; Kuleshov, S. V.] Univ Tecn Federico Santa Maria, Valparaiso, Chile. [Anderson, M. D.; Ireland, D. G.; Lewis, S.; Livingston, K.; MacGregor, I. J. D.; McKinnon, B.; Montgomery, R. A.; Phillips, J. J.; Protopopescu, D.; Rosner, G.; Smith, G. D.; Sokhan, D.] Univ Glasgow, Glasgow G12 8QQ, Lanark, Scotland. [Hanretty, C.; Keller, D.; Tkachenko, S.; Zhao, Z. W.] Univ Virginia, Charlottesville, VA 22901 USA. [Griffioen, K. A.] Coll William & Mary, Williamsburg, VA 23187 USA. [Dashyan, N.; Gevorgyan, N.; Hakobyan, H.; Voskanyan, H.] Yerevan Phys Inst, Yerevan 375036, Armenia. RP Moriya, K (reprint author), Indiana Univ, Bloomington, IN 47405 USA. EM schumacher@cmu.edu RI Celentano, Andrea/J-6190-2012; Adikaram, D/H-7128-2016; Brooks, William/C-8636-2013; Ishkhanov, Boris/E-1431-2012; Schumacher, Reinhard/K-6455-2013; MacGregor, Ian/D-4072-2011; D'Angelo, Annalisa/A-2439-2012; Meyer, Curtis/L-3488-2014; Lu, Haiyun/B-4083-2012; Ireland, David/E-8618-2010; Sabatie, Franck/K-9066-2015; Osipenko, Mikhail/N-8292-2015; Zhang, Jixie/A-1461-2016; Adikaram, Dasuni/D-1539-2016 OI Celentano, Andrea/0000-0002-7104-2983; Bono, Jason/0000-0002-3018-714X; Bellis, Matthew/0000-0002-6353-6043; Brooks, William/0000-0001-6161-3570; Schumacher, Reinhard/0000-0002-3860-1827; D'Angelo, Annalisa/0000-0003-3050-4907; Meyer, Curtis/0000-0001-7599-3973; Ireland, David/0000-0001-7713-7011; Sabatie, Franck/0000-0001-7031-3975; Osipenko, Mikhail/0000-0001-9618-3013; FU DOE [DE-FG02-87ER40315]; United States Department of Energy [DE-AC05-84ER40150]; National Science Foundation; United Kingdom's Science and Technology Facilities Council (STFC) FX We acknowledge the outstanding efforts of the staff of the Accelerator and Physics Divisions at Jefferson Lab that made this experiment possible. The work of the Medium Energy Physics group at Carnegie Mellon University was supported by DOE grant DE-FG02-87ER40315. The Southeastern Universities Research Association (SURA) operated the Thomas Jefferson National Accelerator Facility for the United States Department of Energy under contract DE-AC05-84ER40150. Support was also provided by the National Science Foundation and the United Kingdom's Science and Technology Facilities Council (STFC). NR 43 TC 29 Z9 29 U1 0 U2 16 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD OCT 7 PY 2013 VL 88 IS 4 AR 045201 DI 10.1103/PhysRevC.88.045201 PG 20 WC Physics, Nuclear SC Physics GA 233ME UT WOS:000325572000005 ER PT J AU Cheng, BL Kwan, TJT Wang, YM Batha, SH AF Cheng, Baolian Kwan, Thomas J. T. Wang, Yi-Ming Batha, Steven H. TI Scaling laws for ignition at the National Ignition Facility from first principles SO PHYSICAL REVIEW E LA English DT Article ID CONFINEMENT FUSION-TARGETS; ENERGY; SHELLS AB We have developed an analytical physics model from fundamental physics principles and used the reduced one-dimensional model to derive a thermonuclear ignition criterion and implosion energy scaling laws applicable to inertial confinement fusion capsules. The scaling laws relate the fuel pressure and the minimum implosion energy required for ignition to the peak implosion velocity and the equation of state of the pusher and the hot fuel. When a specific low-entropy adiabat path is used for the cold fuel, our scaling laws recover the ignition threshold factor dependence on the implosion velocity, but when a high-entropy adiabat path is chosen, the model agrees with recent measurements. C1 [Cheng, Baolian; Kwan, Thomas J. T.; Wang, Yi-Ming; Batha, Steven H.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Cheng, BL (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA. EM bcheng@lanl.gov FU US Department of Energy by the Los Alamos National Laboratory [W-7405-ENG-36] FX The authors are grateful to D. Clark, C. Cerjan, S. Haan, J. Nuckolls, and the LLNL NIC Team for valuable comments and sharing data and calculations, to J. Mercer-Smith for useful discussions, and to C. S. Carmer for help with the manuscript. This work was performed under the auspices of the US Department of Energy by the Los Alamos National Laboratory under Contract No. W-7405-ENG-36. NR 14 TC 6 Z9 6 U1 2 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1539-3755 EI 1550-2376 J9 PHYS REV E JI Phys. Rev. E PD OCT 7 PY 2013 VL 88 IS 4 AR 041101 DI 10.1103/PhysRevE.88.041101 PG 4 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA 230XL UT WOS:000325376600002 PM 24229109 ER PT J AU Jayasekara, W Lee, Y Pandey, A Tucker, GS Sapkota, A Lamsal, J Calder, S Abernathy, DL Niedziela, JL Harmon, BN Kreyssig, A Vaknin, D Johnston, DC Goldman, AI McQueeney, RJ AF Jayasekara, W. Lee, Y. Pandey, Abhishek Tucker, G. S. Sapkota, A. Lamsal, J. Calder, S. Abernathy, D. L. Niedziela, J. L. Harmon, B. N. Kreyssig, A. Vaknin, D. Johnston, D. C. Goldman, A. I. McQueeney, R. J. TI Stripe Antiferromagnetic Spin Fluctuations in SrCo2As2 SO PHYSICAL REVIEW LETTERS LA English DT Article AB Inelastic neutron scattering measurements of paramagnetic SrCo2As2 at T = 5 K reveal antiferromagnetic (AFM) spin fluctuations that are peaked at a wave vector of Q(AFM) = (1/2, 1/2, 1) and possess a large energy scale. These stripe spin fluctuations are similar to those found in AFe(2)As(2) compounds, where spin-density wave AFM is driven by Fermi surface nesting between electron and hole pockets separated by Q(AFM). SrCo2As2 has a more complex Fermi surface and band-structure calculations indicate a potential instability toward either a ferromagnetic or stripe AFM ground state. The results suggest that stripe AFM magnetism is a general feature of both iron and cobalt-based arsenides and the search for spin fluctuation-induced unconventional superconductivity should be expanded to include cobalt-based compounds. C1 [Jayasekara, W.; Lee, Y.; Pandey, Abhishek; Tucker, G. S.; Sapkota, A.; Lamsal, J.; Harmon, B. N.; Kreyssig, A.; Vaknin, D.; Johnston, D. C.; Goldman, A. I.; McQueeney, R. J.] Ames Lab, Ames, IA 50011 USA. [Jayasekara, W.; Lee, Y.; Pandey, Abhishek; Tucker, G. S.; Sapkota, A.; Lamsal, J.; Harmon, B. N.; Kreyssig, A.; Vaknin, D.; Johnston, D. C.; Goldman, A. I.; McQueeney, R. J.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Calder, S.; Abernathy, D. L.; Niedziela, J. L.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Jayasekara, W (reprint author), Ames Lab, Ames, IA 50011 USA. RI Tucker, Gregory/L-9357-2013; BL18, ARCS/A-3000-2012; Abernathy, Douglas/A-3038-2012; Pandey, Abhishek /M-5679-2015; McQueeney, Robert/A-2864-2016; Vaknin, David/B-3302-2009; OI Tucker, Gregory/0000-0002-2787-8054; Abernathy, Douglas/0000-0002-3533-003X; Pandey, Abhishek /0000-0003-2839-1720; McQueeney, Robert/0000-0003-0718-5602; Vaknin, David/0000-0002-0899-9248; Calder, Stuart/0000-0001-8402-3741 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-AC02-07CH11358]; U.S. Department of Energy, Office of Basic Energy Sciences, Scientific User Facilities Division FX The authors would like to thank P. C. Canfield, R. M. Fernandes, A. Kaminski, and A. S. Sefat for useful discussions. The work at Ames Laboratory was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, under Contract No. DE-AC02-07CH11358. Work at Oak Ridge National Laboratory is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Scientific User Facilities Division. NR 30 TC 21 Z9 21 U1 6 U2 50 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD OCT 7 PY 2013 VL 111 IS 15 AR 157001 DI 10.1103/PhysRevLett.111.157001 PG 5 WC Physics, Multidisciplinary SC Physics GA 230VO UT WOS:000325371500010 PM 24160618 ER PT J AU Wang, WB Jiang, T Gardner, S AF Wang, Wei-Bung Jiang, Tao Gardner, Shea TI Detection of Homologous Recombination Events in Bacterial Genomes SO PLOS ONE LA English DT Article ID MULTIPLE ALIGNMENT; SMALLPOX; EVOLUTIONARY; DIVERSITY; SEQUENCE; VIRUS; TREES AB We study the detection of mutations, sequencing errors, and homologous recombination events (HREs) in a set of closely related microbial genomes. We base the model on single nucleotide polymorphisms (SNPs) and break the genomes into blocks to handle the rearrangement problem. Then we apply a dynamic programming algorithm to model whether changes within each block are likely a result of mutations, sequencing errors, or HREs. Results from simulation experiments show that we can detect 31%-61% of HREs and the precision of our detection is about 48%-90% depending on the rates of mutation and missing data. The HREfinder software for predicting HREs in a set of whole genomes is available as open source (http://sourceforge.net/projects/hrefinder/). C1 [Wang, Wei-Bung; Jiang, Tao] Univ Calif Riverside, Dept Comp Sci, Riverside, CA 92521 USA. [Gardner, Shea] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Gardner, S (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM Gardner26@llnl.gov FU United States Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; National Institutes of Health [2R01LM008991] FX This work was performed under the auspices of the United States Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344 and was also partially funded by grant National Institutes of Health 2R01LM008991. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 28 TC 0 Z9 0 U1 1 U2 11 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD OCT 7 PY 2013 VL 8 IS 10 AR e75230 DI 10.1371/journal.pone.0075230 PG 14 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 232NS UT WOS:000325501300023 PM 24116030 ER PT J AU Andersson, N Baker, J Belczynski, K Bernuzzi, S Berti, E Cadonati, L Cerda-Duran, P Clark, J Favata, M Finn, LS Fryer, C Giacomazzo, B Gonzalez, JA Hendry, M Heng, IS Hild, S Johnson-McDaniel, N Kalmus, P Klimenko, S Kobayashi, S Kokkotas, K Laguna, P Lehner, L Levin, J Liebling, S MacFadyen, A Mandel, I Marka, S Marka, Z Neilsen, D O'Brien, P Perna, R Read, J Reisswig, C Rodriguez, C Ruffert, M Schnetter, E Searle, A Shawhan, P Shoemaker, D Soderberg, A Sperhake, U Sutton, P Tanvir, N Was, M Whitcomb, S AF Andersson, Nils Baker, John Belczynski, Krzystof Bernuzzi, Sebastiano Berti, Emanuele Cadonati, Laura Cerda-Duran, Pablo Clark, James Favata, Marc Finn, Lee Samuel Fryer, Chris Giacomazzo, Bruno Antonio Gonzalez, Jose Hendry, Martin Heng, Ik Siong Hild, Stefan Johnson-McDaniel, Nathan Kalmus, Peter Klimenko, Sergei Kobayashi, Shiho Kokkotas, Kostas Laguna, Pablo Lehner, Luis Levin, Janna Liebling, Steve MacFadyen, Andrew Mandel, Ilya Marka, Szabolcs Marka, Zsuzsa Neilsen, David O'Brien, Paul Perna, Rosalba Read, Jocelyn Reisswig, Christian Rodriguez, Carl Ruffert, Max Schnetter, Erik Searle, Antony Shawhan, Peter Shoemaker, Deirdre Soderberg, Alicia Sperhake, Ulrich Sutton, Patrick Tanvir, Nial Was, Michal Whitcomb, Stan TI The transient gravitational-wave sky SO CLASSICAL AND QUANTUM GRAVITY LA English DT Review ID GAMMA-RAY BURSTS; CORE-COLLAPSE SUPERNOVAE; MASS BLACK-HOLES; DIFFERENTIALLY ROTATING STARS; ACCRETING NEUTRON-STARS; ARMED SPIRAL INSTABILITY; POLOIDAL MAGNETIC-FIELDS; BAR-MODE INSTABILITY; EARLY WARNING SYSTEM; SPIN-DOWN LIMIT AB Interferometric detectors will very soon give us an unprecedented view of the gravitational-wave sky, and in particular of the explosive and transient Universe. Now is the time to challenge our theoretical understanding of short-duration gravitational-wave signatures from cataclysmic events, their connection to more traditional electromagnetic and particle astrophysics, and the data analysis techniques that will make the observations a reality. This paper summarizes the state of the art, future science opportunities, and current challenges in understanding gravitational-wave transients. C1 [Andersson, Nils] Univ Southampton, Sch Math, Southampton SO17 1BJ, Hants, England. [Baker, John] NASA GSFC, Gravitat Phys Lab, Greenbelt, MD 20771 USA. [Belczynski, Krzystof] Univ Warsaw, Astron Observ, PL-00478 Warsaw, Poland. [Belczynski, Krzystof] Univ Texas Brownsville, Ctr Gravitat Wave Astron, Brownsville, TX 78520 USA. [Bernuzzi, Sebastiano; Johnson-McDaniel, Nathan] Univ Jena, Inst Theoret Phys, D-07743 Jena, Germany. [Berti, Emanuele] Univ Mississippi, Dept Phys & Astron, University, MS 38677 USA. [Berti, Emanuele; Reisswig, Christian; Sperhake, Ulrich] CALTECH, Pasadena, CA 91125 USA. [Cadonati, Laura; Clark, James] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Cerda-Duran, Pablo] Univ Valencia, Dept Astron & Astrofis, E-46100 Burjassot, Spain. [Favata, Marc] Montclair State Univ, Montclair, NJ 07043 USA. [Finn, Lee Samuel] Penn State Univ, Dept Phys, University Pk, PA 16802 USA. [Finn, Lee Samuel] Penn State Univ, Dept Astron & Astrophys, University Pk, PA 16802 USA. [Fryer, Chris] Los Alamos Natl Lab, CCS 2, Los Alamos, NM 87545 USA. [Giacomazzo, Bruno; Perna, Rosalba] Univ Colorado, JILA, Boulder, CO 80309 USA. [Giacomazzo, Bruno; Perna, Rosalba] NIST, Boulder, CO 80309 USA. [Antonio Gonzalez, Jose] Univ Michoacana, Inst Fis & Matemat, Morelia 58040, Michoacan, Mexico. [Hendry, Martin; Heng, Ik Siong] Univ Glasgow, Sch Phys & Astron, SUPA, Glasgow G12 8QQ, Lanark, Scotland. [Hild, Stefan] Univ Glasgow, Inst Gravitat Res, Glasgow G12 8QQ, Lanark, Scotland. [Kalmus, Peter; Searle, Antony; Whitcomb, Stan] CALTECH, LIGO Lab, Pasadena, CA 91125 USA. [Klimenko, Sergei] Univ Florida, Gainesville, FL 32611 USA. [Kobayashi, Shiho] Liverpool John Moores Univ, Astrophys Res Inst, Birkenhead CH41 1LD, Merseyside, England. [Kokkotas, Kostas] Univ Tubingen, IAAT, D-72076 Tubingen, Germany. [Laguna, Pablo; Shoemaker, Deirdre] Georgia Inst Technol, Sch Phys, Atlanta, GA 30332 USA. [Lehner, Luis; Schnetter, Erik] Perimeter Inst Theoret Phys, Waterloo, ON, Canada. [Levin, Janna] Columbia Univ Barnard Coll, Dept Phys & Astron, New York, NY 10027 USA. [Liebling, Steve] Long Isl Univ, Brookville, NY 11548 USA. [MacFadyen, Andrew] New York Univ, Dept Phys, New York, NY 10003 USA. [Mandel, Ilya] Univ Birmingham, Sch Phys & Astron, Birmingham B15 2TT, W Midlands, England. [Marka, Szabolcs] Columbia Univ, Dept Phys, New York, NY 10027 USA. [Marka, Zsuzsa] Columbia Univ, Columbia Astrophys Lab, New York, NY 10027 USA. [Neilsen, David] Brigham Young Univ, Dept Phys & Astron, Provo, UT 84602 USA. [O'Brien, Paul; Tanvir, Nial] Univ Leicester, Dept Phys & Astron, Leicester LE1 7RH, Leics, England. [Read, Jocelyn] Calif State Univ Fullerton, Dept Phys, Fullerton, CA 92831 USA. [Rodriguez, Carl] Northwestern Univ, Dept Phys & Astron, Evanston, IL 60208 USA. [Ruffert, Max] Univ Edinburgh, Sch Math, Edinburgh EH16 5JN, Midlothian, Scotland. [Ruffert, Max] Univ Edinburgh, Maxwell Inst, Edinburgh EH16 5JN, Midlothian, Scotland. [Schnetter, Erik] Univ Guelph, Dept Phys, Guelph, ON N1G 2W1, Canada. [Schnetter, Erik] Louisiana State Univ, Ctr Computat & Technol, Baton Rouge, LA 70803 USA. [Shawhan, Peter] Univ Maryland, College Pk, MD 20742 USA. [Soderberg, Alicia] Harvard Smithsonian Ctr Astrophys, Cambridge, MA 02138 USA. [Sperhake, Ulrich] Ctr Math Sci, DAMTP, Cambridge CB3 0WA, England. [Sperhake, Ulrich] CENTRA IST, Lisbon, Portugal. [Sutton, Patrick] Cardiff Univ, Sch Phys & Astron, Cardiff CF24 3AA, S Glam, Wales. [Was, Michal] Max Planck Inst Gravitat Phys, Albert Einstein Inst, D-30167 Hannover, Germany. RP Andersson, N (reprint author), Univ Southampton, Sch Math, Southampton SO17 1BJ, Hants, England. EM plaguna@gatech.edu RI Hild, Stefan/A-3864-2010; Kokkotas, Kostas/B-7878-2010; Cerda-Duran, Pablo/D-7857-2015; Finn, Lee Samuel/A-3452-2009; Neilsen, David/J-4862-2015; Berti, Emanuele/C-9331-2016; Giacomazzo, Bruno/I-8088-2012; OI Kokkotas, Kostas/0000-0001-6048-2919; Cerda-Duran, Pablo/0000-0003-4293-340X; Finn, Lee Samuel/0000-0002-3937-0688; Neilsen, David/0000-0002-6142-5542; Berti, Emanuele/0000-0003-0751-5130; Giacomazzo, Bruno/0000-0002-6947-4023; Schnetter, Erik/0000-0002-4518-9017; Reisswig, Christian/0000-0001-6855-9351; MacFadyen, Andrew/0000-0002-0106-9013; Mandel, Ilya/0000-0002-6134-8946 FU National Science Foundation [0946361, 1231548, PHY-0847182, PHY-1055103, PHY-0653550, PHY-0955773, PHY-0653462, CBET-0940924, PHY-0969857, 0903973, 1205864, PHY-0925345, PHY-0955825]; Australian Research Council; International Science Linkages program of the Commonwealth of Australia; Council of Scientific and Industrial Research of India; Istituto Nazionale di Fisica Nucleare of Italy; Spanish Ministerio de Educacion y Ciencia; Conselleria d'Economia, Hisenda i Innovacio of the Govern de les Illes Balears; Royal Society; Scottish Funding Council; Scottish Universities Physics Alliance; National Aeronautics and Space Administration; Carnegie Trust; Leverhulme Trust; David and Lucile Packard Foundation; Research Corporation; Alfred P Sloan Foundation; NSF [PHY11-25915, HRD 1242090, AST-1009396]; Columbia University in the City of New York; NASA [NNX09AV06A, NNX12AO67G]; German Science Foundation [SFB/TR7]; NSERC; Industry Canada; Province of Ontario through the Ministry of Research and Innovation; Spanish Ministerio de Educacion y Ciencia [AYA 2010-21097-C03-01]; Generalitat Valenciana [PROMETEO-2009-103]; ERC [CAMAP-259276]; US Department of Energy [W-7405-ENG-36] FX The 'Gravitational Wave Bursts' workshops in Chichen-Itza, Mexico (9-1 December 2009) and Tobermory, Scotland (29-31 May 2012) were supported by National Science Foundation grant numbers 0946361 and 1231548. The authors gratefully acknowledge the support of the United States National Science Foundation for the construction and operation of the LIGO Laboratory and the Science and Technology Facilities Council of the United Kingdom, the Max-Planck-Society, and the State of Niedersachsen/Germany for support of the construction and operation of the GEO600 detector. The authors also gratefully acknowledge the support of the research by these agencies and by the Australian Research Council, the International Science Linkages program of the Commonwealth of Australia, the Council of Scientific and Industrial Research of India, the Istituto Nazionale di Fisica Nucleare of Italy, the Spanish Ministerio de Educacion y Ciencia, the Conselleria d'Economia, Hisenda i Innovacio of the Govern de les Illes Balears, the Royal Society, the Scottish Funding Council, the Scottish Universities Physics Alliance, The National Aeronautics and Space Administration, the Carnegie Trust, the Leverhulme Trust, the David and Lucile Packard Foundation, the Research Corporation, and the Alfred P Sloan Foundation. We thank the Kavli Institute for Theoretical Physics at UC-Santa Barbara, supported in part by NSF grant PHY11-25915, for hosting the workshop 'Chirps, Mergers and Explosions: The Final Moments of Coalescing Compact Binaries.' The Columbia Experimental Gravity group is grateful for the generous support from Columbia University in the City of New York and from the National Science Foundation under cooperative agreement PHY-0847182. E.B. is supported by National Science Foundation through CAREER Award Number PHY-1055103. KB acknowledges NASA grant number NNX09AV06A and NSF grant numbers HRD 1242090 awarded to the Center for Gravitational Wave Astronomy, UTB. SB and KK acknowledge support from the German Science Foundation SFB/TR7 'Gravitational Wave Astronomy.' LC acknowledges National Science Foundation grant numbers PHY-0653550 and PHY-0955773. LL was supported in part by an NSERC through discovery grant. Research at Perimeter Institute is supported through Industry Canada and by the Province of Ontario through the Ministry of Research and Innovation. PCD acknowledges Spanish Ministerio de Educacion y Ciencia grant number AYA 2010-21097-C03-01, Generalitat Valenciana grant number PROMETEO-2009-103 and ERC starting grant number CAMAP-259276. The work of CF is under the auspices of the US Department of Energy, and supported by its contract W-7405-ENG-36 to Los Alamos National Laboratory. LSF acknowledges National Science Foundation grant numbers PHY-0653462, CBET-0940924 and PHY-0969857. BG and RP acknowledge support from NSF grant number AST-1009396 and NASA grant number NNX12AO67G. PL acknowledges National Science Foundation grant numbers 0903973 and 1205864. DMS acknowledges National Science Foundation grant numbers PHY-0925345 and PHY-0955825. We wish to thank Christian Ott and Harald Pfeiffer for useful contributions to this review. NR 421 TC 24 Z9 24 U1 1 U2 22 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0264-9381 EI 1361-6382 J9 CLASSICAL QUANT GRAV JI Class. Quantum Gravity PD OCT 7 PY 2013 VL 30 IS 19 AR 193002 DI 10.1088/0264-9381/30/19/193002 PG 45 WC Astronomy & Astrophysics; Physics, Multidisciplinary; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 223PW UT WOS:000324819900002 ER PT J AU DeGottardi, W Thakurathi, M Vishveshwara, S Sen, D AF DeGottardi, Wade Thakurathi, Manisha Vishveshwara, Smitha Sen, Diptiman TI Majorana fermions in superconducting wires: Effects of long-range hopping, broken time-reversal symmetry, and potential landscapes SO PHYSICAL REVIEW B LA English DT Article ID TOPOLOGICAL INSULATORS; MAGNETIC-FIELD; LOCALIZATION; NANOWIRE; MODEL; CONDUCTANCE; SIGNATURE; DISORDER; ELECTRON; SYSTEMS AB We present a comprehensive study of two of the most experimentally relevant extensions of Kitaev's spinless model of a one-dimensional p-wave superconductor: those involving (i) longer-range hopping and superconductivity and (ii) inhomogeneous potentials. We commence with a pedagogical review of the spinless model and, as a means of characterizing topological phases exhibited by the systems studied here, we introduce bulk topological invariants as well as those derived from an explicit consideration of boundary modes. In time-reversal symmetric systems, we find that the longer range hopping leads to topological phases characterized by multiple Majorana modes. In particular, we investigate a spin model that respects a duality and maps to a fermionic model with multiple Majorana modes; we highlight the connection between these topological phases and the broken symmetry phases in the original spin model. In the presence of time-reversal symmetry breaking terms, we show that the topological phase diagram is characterized by an extended gapless regime. For the case of inhomogeneous potentials, we explore phase diagrams of periodic, quasiperiodic, and disordered systems. We present a detailed mapping between normal state localization properties of such systems and the topological phases of the corresponding superconducting systems. This powerful tool allows us to leverage the analyses of Hofstadter's butterfly and the vast literature on Anderson localization to the question of Majorana modes in superconducting quasiperiodic and disordered systems, respectively. We briefly touch upon the synergistic effects that can be expected in cases where long-range hopping and disorder are both present. C1 [DeGottardi, Wade] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Thakurathi, Manisha; Sen, Diptiman] Indian Inst Sci, Ctr High Energy Phys, Bangalore 560012, Karnataka, India. [Vishveshwara, Smitha] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. RP DeGottardi, W (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. FU NSF [DMR 0644022-CAR]; UChicago Argonne, LLC, operator of Argonne National Laboratory [DE-AC02-06CH11357]; CSIR, India; DST, India [SR/S2/JCB-44/2010]; Simons Foundation [229047]; US Department of Energy [DE-FG02-07ER46453] FX For support, W.D. thanks the NSF under Grant DMR 0644022-CAR and UChicago Argonne, LLC, operator of Argonne National Laboratory, under Contract No. DE-AC02-06CH11357; M.T. thanks CSIR, India; D.S. thanks DST, India under Project No. SR/S2/JCB-44/2010; S.V. thanks the Simons Foundation under Grant No. 229047 and the US Department of Energy, under Award No. DE-FG02-07ER46453. W.D. and S.V. thank the Indian Institute of Science for its generous hospitality at different stages of this work. We are grateful to Ilya Gruzberg, Shinsei Ryu, and Jay Deep Sau for their illuminating comments. NR 82 TC 30 Z9 30 U1 0 U2 21 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD OCT 7 PY 2013 VL 88 IS 16 AR 165111 DI 10.1103/PhysRevB.88.165111 PG 22 WC Physics, Condensed Matter SC Physics GA 232OD UT WOS:000325502400007 ER PT J AU Kim, HC Logan, JM Shpyrko, OG Littlewood, PB Isaacs, ED AF Kim, Hyekyung Clarisse Logan, Jonathan Michael Shpyrko, O. G. Littlewood, P. B. Isaacs, E. D. TI Metastability and microscopic avalanche dynamics in charge-density waves of chromium SO PHYSICAL REVIEW B LA English DT Article ID X-RAY-SCATTERING; DOMAIN-WALLS; Q-VECTOR; FIELD; SUPERCONDUCTORS; SYSTEMS; STATE; ORDER AB We have measured the relaxation of charge-density waves in chromium from out-of-equilibrium states achieved through rapid thermal quenching. Although pinned density waves have been predicted to relax through stick-slip dynamics, in which long-lived metastable states are linked by abrupt rearrangements of the microscopic structure, these microscopic behaviors have not been observed. Using synchrotron x rays, we have measured metastability of the order parameter and microscopic pinning phenomena including an avalanche of the charge-density wave phase. Molecular dynamical simulations based on the Fukuyama-Lee-Rice model show that these behaviors may be attributed to nucleation, pinning, and propagation of phase solitons. C1 [Kim, Hyekyung Clarisse; Logan, Jonathan Michael; Littlewood, P. B.; Isaacs, E. D.] Univ Chicago, Dept Phys, Chicago, IL 60637 USA. [Shpyrko, O. G.] Univ Calif San Diego, Dept Phys, La Jolla, CA 92093 USA. [Littlewood, P. B.; Isaacs, E. D.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Kim, HC (reprint author), Univ Chicago, Dept Phys, Chicago, IL 60637 USA. RI Littlewood, Peter/B-7746-2008; OI Logan, Jonathan/0000-0003-2554-9457 FU US Department of Energy, Office of Science [DE-AC02-06CH11357]; US Department of Energy, Office of Basic Energy Sciences [DE-AC02-06CH11357]; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001805] FX Use of the Advanced Photon Source was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences. We thank beam line scientists A. Sandy, M. Sprung, S. Narayanan, and M. Holt for their expertise and support. Use of the Advanced Photon Source was supported by the US Department of Energy, Office of Science, and Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. Work at the University of California, San Diego was supported by US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-SC0001805. NR 32 TC 2 Z9 2 U1 2 U2 15 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD OCT 7 PY 2013 VL 88 IS 14 AR 140101 DI 10.1103/PhysRevB.88.140101 PG 5 WC Physics, Condensed Matter SC Physics GA 232MP UT WOS:000325498300001 ER PT J AU Rodriguez, EE Sokolov, DA Stock, C Green, MA Sobolev, O Rodriguez-Rivera, JA Cao, H Daoud-Aladine, A AF Rodriguez, E. E. Sokolov, D. A. Stock, C. Green, M. A. Sobolev, O. Rodriguez-Rivera, Jose A. Cao, H. Daoud-Aladine, A. TI Magnetic and structural properties near the Lifshitz point in Fe1+xTe SO PHYSICAL REVIEW B LA English DT Article ID HIGH-TEMPERATURE SUPERCONDUCTIVITY; PHASE-DIAGRAM; FIELD; MNP; SUSCEPTIBILITY; TRANSITIONS; BEHAVIOR; NEUTRON AB We construct a phase diagram of the parent compound Fe1+xTe as a function of interstitial iron x in terms of the electronic, structural, and magnetic properties. For a concentration of x < 10%, Fe1+xTe undergoes a "semimetal" to metal transition at approximately 70 K that is also first-order and coincident with a structural transition from a tetragonal to a monoclinic unit cell. For x approximate to 14%, Fe1+xTe undergoes a second-order phase transition at approximately 58 K corresponding to a semimetal to semimetal transition along with a structural orthorhombic distortion. At a critical concentration of x approximate to 11%, Fe1+xTe undergoes two transitions: the higher-temperature one is a second-order transition to an orthorhombic phase with incommensurate magnetic ordering and temperature-dependent propagation vector, while the lower-temperature one corresponds to nucleation of a monoclinic phase with a nearly commensurate magnetic wave vector. While both structural and magnetic transitions display similar critical behavior for x < 10% and near the critical concentration of x approximate to 11%, samples with large interstitial iron concentrations show a marked deviation between the critical response indicating a decoupling of the order parameters. Analysis of temperature dependent inelastic neutron data reveals incommensurate magnetic fluctuations throughout the Fe1+xTe phase diagram are directly connected to the "semiconductor"-like resistivity above T-N and implicates scattering from spin fluctuations as the primary reason for the semiconducting or poor metallic properties. The results suggest that doping driven Fermi surface nesting maybe the origin of the gapless and incommensurate spin response at large interstitial concentrations. C1 [Rodriguez, E. E.] Univ Maryland, Dept Chem Biochem, College Pk, MD 20742 USA. [Sokolov, D. A.; Stock, C.] Univ Edinburgh, Sch Phys & Astron, Edinburgh EH9 3JZ, Midlothian, Scotland. [Green, M. A.] Univ Kent, Sch Phys Sci, Canterbury CT2 7NH, Kent, England. [Sobolev, O.] FRM2 Garching, Forsch Neutronenquelle Heinz Maier Leibnitz, D-85747 Garching, Germany. [Rodriguez-Rivera, Jose A.] NIST, NIST Ctr Neutron Res, Gaithersburg, MD 20889 USA. [Rodriguez-Rivera, Jose A.] Univ Maryland, Dept Mat Sci, College Pk, MD 20742 USA. [Cao, H.] Oak Ridge Natl Lab, Neutron Scattering Sci Div, Oak Ridge, TN 37831 USA. [Daoud-Aladine, A.] Rutherford Appleton Lab, ISIS Facil, Didcot OX11 0QX, Oxon, England. RP Rodriguez, EE (reprint author), Univ Maryland, Dept Chem Biochem, College Pk, MD 20742 USA. RI Sokolov, D/G-7755-2011; Rodriguez-Rivera, Jose/A-4872-2013; Cao, Huibo/A-6835-2016; Sobolev, Oleg/P-5983-2016 OI Rodriguez-Rivera, Jose/0000-0002-8633-8314; Cao, Huibo/0000-0002-5970-4980; FU NRC, Department of Commerce; National Science Foundation [DMR-0944772]; Carnegie Trust for the Universities of Scotland; Royal Society of Edinburgh FX Work at NIST, Oak Ridge, and ISIS was funded by the NRC, Department of Commerce, and by the National Science Foundation under Agreement No. DMR-0944772. Work performed through the University of Edinburgh was funded by the Carnegie Trust for the Universities of Scotland and the Royal Society of Edinburgh. We are grateful to N. C. Maliszewskyj for expert technical support for experiments performed on MACS. NR 97 TC 21 Z9 21 U1 4 U2 51 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-0121 J9 PHYS REV B JI Phys. Rev. B PD OCT 7 PY 2013 VL 88 IS 16 AR 165110 DI 10.1103/PhysRevB.88.165110 PG 15 WC Physics, Condensed Matter SC Physics GA 232OD UT WOS:000325502400006 ER PT J AU Lenaghan, SC Burris, JN Chourey, K Huang, YJ Xia, LJ Lady, B Sharma, R Pan, CL LeJeune, Z Foister, S Hettich, RL Stewart, CN Zhang, MJ AF Lenaghan, Scott C. Burris, Jason N. Chourey, Karuna Huang, Yujian Xia, Lijin Lady, Belinda Sharma, Ritin Pan, Chongle LeJeune, Zorabel Foister, Shane Hettich, Robert L. Stewart, C. Neal, Jr. Zhang, Mingjun TI Isolation and chemical analysis of nanoparticles from English ivy (Hedera helix L.) SO JOURNAL OF THE ROYAL SOCIETY INTERFACE LA English DT Article DE bioadhesive; nanoparticles; nanocomposite; English ivy ID ADHESIVE; CHROMATOGRAPHY; PARTICLES; TENDRIL; MUSSEL AB Bio-inspiration for novel adhesive development has drawn increasing interest in recent years with the discovery of the nanoscale morphology of the gecko footpad and mussel adhesive proteins. Similar to these animal systems, it was discovered that English ivy (Hedera helix L.) secretes a high strength adhesive containing uniform nanoparticles. Recent studies have demonstrated that the ivy nanoparticles not only contribute to the high strength of this adhesive, but also have ultraviolet (UV) protective abilities, making them ideal for sunscreen and cosmetic fillers, and may be used as nanocarriers for drug delivery. To make these applications a reality, the chemical nature of the ivy nanoparticles must be elucidated. In the current work, a method was developed to harvest bulk ivy nanoparticles from an adventitious root culture system, and the chemical composition of the nanoparticles was analysed. UV/visible spectroscopy, inductively coupled plasma mass spectrometry, Fourier transforminfrared spectroscopy and electrophoresis were used in this study to identify the chemical nature of the ivy nanoparticles. Based on this analysis, we conclude that the ivy nanoparticles are proteinaceous. C1 [Lenaghan, Scott C.; Huang, Yujian; Xia, Lijin; LeJeune, Zorabel; Zhang, Mingjun] Univ Tennessee, Dept Mech Aerosp & Biomed Engn, Knoxville, TN 37996 USA. [Burris, Jason N.; Stewart, C. Neal, Jr.] Univ Tennessee, Dept Plant Sci, Knoxville, TN 37996 USA. [Lady, Belinda; Foister, Shane] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Sharma, Ritin] Univ Tennessee, UT ORNL Grad Sch Genome Sci & Technol, Knoxville, TN 37996 USA. [Chourey, Karuna; Sharma, Ritin; Hettich, Robert L.] Oak Ridge Natl Lab, Div Chem Sci, Organ & Biol Mass Spectrometry Grp, Oak Ridge, TN 37831 USA. [Pan, Chongle] Oak Ridge Natl Lab, Comp Sci Math & BioSci Div, Oak Ridge, TN 37831 USA. RP Zhang, MJ (reprint author), Univ Tennessee, Dept Mech Aerosp & Biomed Engn, Knoxville, TN 37996 USA. EM mjzhang@utk.edu RI Huang, Yujian/B-2085-2016; Hettich, Robert/N-1458-2016; OI Huang, Yujian/0000-0001-8543-0269; Hettich, Robert/0000-0001-7708-786X; , /0000-0002-9216-3813; Lenaghan, Scott/0000-0002-7539-1726 FU Army Research Office [W911NF-10-1-0114]; National Science Foundation (CMMI) [1029953]; National Science Foundation (CBET) [0965877]; Genome Science and Technology Graduate School at UT-Knoxville; US Department of Energy, Biological and Environmental Research Division, Genome Sciences Program FX This research is partially sponsored by the Army Research Office (W911NF-10-1-0114) and the National Science Foundation (CMMI, 1029953; CBET, 0965877). The authors are grateful for the support. R.S. acknowledges graduate stipend support from the Genome Science and Technology Graduate School at UT-Knoxville. Financial support to K.C., C.P. and R.L.H. was provided by the US Department of Energy, Biological and Environmental Research Division, Genome Sciences Program. Oak Ridge National Laboratory is managed by University of Tennessee-Battelle LLC for the Department of Energy. NR 29 TC 5 Z9 5 U1 6 U2 35 PU ROYAL SOC PI LONDON PA 6-9 CARLTON HOUSE TERRACE, LONDON SW1Y 5AG, ENGLAND SN 1742-5689 EI 1742-5662 J9 J R SOC INTERFACE JI J. R. Soc. Interface PD OCT 6 PY 2013 VL 10 IS 87 AR 20130392 DI 10.1098/rsif.2013.0392 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 298BG UT WOS:000330298300002 PM 23883948 ER PT J AU Laverock, B Kitidis, V Tait, K Gilbert, JA Osborn, AM Widdicombe, S AF Laverock, B. Kitidis, V. Tait, K. Gilbert, J. A. Osborn, A. M. Widdicombe, S. TI Bioturbation determines the response of benthic ammonia-oxidizing microorganisms to ocean acidification SO PHILOSOPHICAL TRANSACTIONS OF THE ROYAL SOCIETY B-BIOLOGICAL SCIENCES LA English DT Article DE ocean acidification; ammonia oxidation; marine sediments; bioturbation; Upogebia deltaura ID COASTAL MARINE-SEDIMENTS; ORGANIC-MATTER DIAGENESIS; UPOGEBIA-DELTAURA; DEEP-SEA; SEAWATER ACIDIFICATION; NITRIFYING BACTERIA; CACO3 DISSOLUTION; NITROGEN-CYCLE; NUTRIENT FLUX; MUD-SHRIMP AB Ocean acidification (OA), caused by the dissolution of increasing concentrations of atmospheric carbon dioxide (CO2) in seawater, is projected to cause significant changes to marine ecology and biogeochemistry. Potential impacts on the microbially driven cycling of nitrogen are of particular concern. Specifically, under seawater pH levels approximating future OA scenarios, rates of ammonia oxidation (the rate-limiting first step of the nitrification pathway) have been shown to dramatically decrease in seawater, but not in underlying sediments. However, no prior study has considered the interactive effects of microbial ammonia oxidation and macrofaunal bioturbation activity, which can enhance nitrogen transformation rates. Using experimental mesocosms, we investigated the responses to OA of ammonia oxidizing microorganisms inhabiting surface sediments and sediments within burrow walls of the mud shrimp Upogebia deltaura. Seawater was acidified to one of four target pH values (pH(T) 7.90, 7.70, 7.35 and 6.80) in comparison with a control (pH(T) 8.10). At pH(T) 8.10, ammonia oxidation rates in burrow wall sediments were, on average, fivefold greater than in surface sediments. However, at all acidified pH values (pH <= 7.90), ammonia oxidation rates in burrow sediments were significantly inhibited (by 79-97%; p < 0.01), whereas rates in surface sediments were unaffected. Both bacterial and archaeal abundances increased significantly as pHT declined; by contrast, relative abundances of bacterial and archaeal ammonia oxidation (amoA) genes did not vary. This research suggests that OA could cause substantial reductions in total benthic ammonia oxidation rates in coastal bioturbated sediments, leading to corresponding changes in coupled nitrogen cycling between the benthic and pelagic realms. C1 [Laverock, B.; Kitidis, V.; Tait, K.; Widdicombe, S.] Plymouth Marine Lab, Plymouth PL1 3DH, Devon, England. [Laverock, B.; Osborn, A. M.] Univ Sheffield, Dept Anim & Plant Sci, Sheffield S10 2TN, S Yorkshire, England. [Laverock, B.] Univ Western Australia, Sch Plant Biol, Crawley, WA 6009, Australia. [Laverock, B.] Univ Western Australia, UWA Oceans Inst, Crawley, WA 6009, Australia. [Gilbert, J. A.] Argonne Natl Lab, Inst Genom & Syst Biol, Argonne, IL 60439 USA. [Gilbert, J. A.] Univ Chicago, Dept Ecol & Evolut, Chicago, IL 60637 USA. [Osborn, A. M.] Univ Hull, Dept Biol Sci, Kingston Upon Hull HU6 7RX, N Humberside, England. RP Laverock, B (reprint author), Plymouth Marine Lab, Prospect Pl, Plymouth PL1 3DH, Devon, England. EM bonnie.laverock@uwa.edu.au RI Osborn, Andrew/F-5466-2015; OI Osborn, Andrew/0000-0002-6433-0581; Kitidis, Vassilis/0000-0003-3949-3802 FU NERC [NE/F008864/1]; NERC FX B.L. acknowledges support from a NERC Algorithm PhD Studentship (NE/F008864/1) and from the NERC-funded programme Oceans 2025 (Theme 3: Coastal and shelf processes). NR 91 TC 9 Z9 9 U1 4 U2 35 PU ROYAL SOC PI LONDON PA 6-9 CARLTON HOUSE TERRACE, LONDON SW1Y 5AG, ENGLAND SN 0962-8436 EI 1471-2970 J9 PHILOS T R SOC B JI Philos. Trans. R. Soc. B-Biol. Sci. PD OCT 5 PY 2013 VL 368 IS 1627 AR UNSP 20120441 DI 10.1098/rstb.2012.0441 PG 13 WC Biology SC Life Sciences & Biomedicine - Other Topics GA AA6QL UT WOS:000331222800004 PM 23980243 ER PT J AU Sheng, X Hanus, R Bauer, A Kessler, MR AF Sheng, Xia Hanus, Riley Bauer, Amy Kessler, Michael R. TI Effect of PEGDE addition on rheological and mechanical properties of bisphenol E cyanate ester SO JOURNAL OF APPLIED POLYMER SCIENCE LA English DT Article DE blends; thermosets; mechanical properties; glass transition; resins ID LAYERED SILICATE NANOCOMPOSITES; EPOXY-RESIN MATRICES; POLYFUNCTIONAL GLYCIDYLETHERS; MOISTURE ABSORPTION; CYANIC ACID; PROCESSABILITY; POLYMERS AB Cyanate esters are a group of resins with exceptional thermal and mechanical properties and are often blended with lower cost epoxy resins. These blends are often brittle, and a toughening method, such as the addition of soft segments, is necessary. Poly(ethylene glycol) diglycidyl ether, or PEGDE, was added to bisphenol E cyanate ester as a toughening agent. PEGDE was added at loadings of 0-30 wt %, and rheological and mechanical properties were analyzed after curing. As PEGDE loading was increased, the gel point increased accordingly while the activation energy of gelation decreased, indicating PEGDE accelerated the gelation process. Dynamic mechanical analysis results indicated a decrease in glass transition temperature as the PEGDE loading increased. Three-point bending tests yielded similar toughness to the neat BECy at low PEGDE loadings, with a dramatic increase at loadings of 25 and 30 wt % PEGDE. (c) 2013 Wiley Periodicals, Inc. J. Appl. Polym. Sci., 2013 C1 [Sheng, Xia; Hanus, Riley; Bauer, Amy; Kessler, Michael R.] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. [Kessler, Michael R.] Iowa State Univ, Dept Mech Engn, Ames, IA 50011 USA. [Kessler, Michael R.] US DOE, Ames Lab, Ames, IA 50011 USA. RP Kessler, MR (reprint author), Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. EM mkessler@iastate.edu RI Kessler, Michael/C-3153-2008; Sheng, Xia/D-5455-2009 OI Kessler, Michael/0000-0001-8436-3447; FU Department of Energy's Science Undergraduate Laboratory Internship program FX Support from the Department of Energy's Science Undergraduate Laboratory Internship program is gratefully acknowledged. NR 23 TC 6 Z9 7 U1 2 U2 42 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0021-8995 J9 J APPL POLYM SCI JI J. Appl. Polym. Sci. PD OCT 5 PY 2013 VL 130 IS 1 BP 463 EP 469 DI 10.1002/app.39118 PG 7 WC Polymer Science SC Polymer Science GA 176LI UT WOS:000321305500055 ER PT J AU Darling, KA Roberts, AJ Mishin, Y Mathaudhu, SN Kecskes, LJ AF Darling, K. A. Roberts, A. J. Mishin, Y. Mathaudhu, S. N. Kecskes, L. J. TI Grain size stabilization of nanocrystalline copper at high temperatures by alloying with tantalum SO JOURNAL OF ALLOYS AND COMPOUNDS LA English DT Article DE Nanocrystalline alloys; Grain-growth; Binary alloys; Stability; Thermal analysis; Immiscible systems ID THERMAL-STABILITY; MICROSTRUCTURAL EVOLUTION; THERMOKINETIC DESCRIPTION; SOLUTE SEGREGATION; TRIPLE JUNCTIONS; GROWTH; CU; SYSTEM; ENERGY; NANOSTRUCTURES AB Nanocrystalline Cu-Ta alloys belong to an emerging class of immiscible materials with potential for high-temperature applications. Differential scanning calorimetry (DSC), Vickers microhardness, transmission and scanning electron microscopy (TEM/SEM), and atomistic simulations have been applied to study the structural evolution in high-energy cryogenically alloyed nanocrystalline Cu-10 at.%Ta. The thermally induced coarsening of the as-milled microstructure was investigated and it was found that the onset of grain growth occurs at temperatures higher than that for pure nanocrystalline Cu. The total heat release associated with grain growth was 0.553 kJ/mol. Interestingly, nanocrystalline Cu-10 at.%Ta maintains a mean grain size (GS) of 167 nm after annealing at 97% of its melting point. The increased microstructural stability is attributed to a combination of thermodynamic and kinetic stabilization effects which, in turn, appear to be controlled by segregation and diffusion of Ta solute atoms along grain boundaries (GBs). The as-milled nanocrystalline Cu-10 at.% Ta exhibits Vickers microhardness values near 5 GPa surpassing the microhardness of conventional pure nanocrystalline Cu by similar to 2.5 GPa. Published by Elsevier B.V. C1 [Darling, K. A.; Kecskes, L. J.] USA, Res Lab, Weap & Mat Res Directorate, Aberdeen Proving Ground, MD 21005 USA. [Roberts, A. J.] USA, ORISE Program, Res Lab, Aberdeen Proving Ground, MD 21005 USA. [Mishin, Y.] George Mason Univ, Dept Phys & Astron, Fairfax, VA 22030 USA. [Mathaudhu, S. N.] USA, Res Lab, Army Res Off, Res Triangle Pk, NC 27709 USA. RP Darling, KA (reprint author), USA, Res Lab, Weap & Mat Res Directorate, Aberdeen Proving Ground, MD 21005 USA. EM kristopher.darling.civ@mail.mil RI Kecskes, Laszlo/F-6880-2014; Mathaudhu, Suveen/B-4192-2009; Mishin, Yuri/P-2020-2015 OI Kecskes, Laszlo/0000-0002-1342-3729; FU Strategic Environmental Research and Development Program, Arlington VA [WP-2139] FX The authors would like to thank the Strategic Environmental Research and Development Program, 901 North Stuart Street, Arlington VA 2203 for funding this effort under Project Number WP-2139. NR 80 TC 34 Z9 35 U1 12 U2 119 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0925-8388 J9 J ALLOY COMPD JI J. Alloy. Compd. PD OCT 5 PY 2013 VL 573 BP 142 EP 150 DI 10.1016/j.jallcom.2013.03.177 PG 9 WC Chemistry, Physical; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Chemistry; Materials Science; Metallurgy & Metallurgical Engineering GA 166VC UT WOS:000320585700023 ER PT J AU Paul, KB Hedge, JM Macherla, C Filer, DL Burgess, E Simmons, SO Crofton, KM Hornung, MW AF Paul, Katie B. Hedge, Joan M. Macherla, Chitralekha Filer, Dayne L. Burgess, Emily Simmons, Steven O. Crofton, Kevin M. Hornung, Michael W. TI Cross-species analysis of thyroperoxidase inhibition by xenobiotics demonstrates conservation of response between pig and rat SO TOXICOLOGY LA English DT Article DE Thyroperoxidase; Thyroid disruption; Interspecies comparison ID FOLLICULAR CELL-PROLIFERATION; THYROID-HORMONE INSUFFICIENCY; IN-VITRO; MATERNAL HYPOTHYROXINEMIA; EARLY-PREGNANCY; DEVELOPMENTAL HYPOTHYROIDISM; DISRUPTING CHEMICALS; NEURONAL MIGRATION; NEONATAL THYROXINE; RADICAL MECHANISM AB Thyroperoxidase (TPO), the enzyme that catalyzes the synthesis of thyroid hormone, is a known target for thyroid-disrupting chemicals. In vivo toxicological evidence supporting TPO-inhibition as one molecular-initiating event that leads to thyroid disruption is derived largely from rat models; however, a significant fraction of research on the inhibition of TPO by xenobiotics has been conducted using porcine TPO. The current work tested the hypothesis that porcine and rat thyroid microsomes exposed to TPO-inhibiting chemicals would demonstrate different responses in a guaiacol oxidation assay. A primary objective of this work is to establish the degree of concordance between rat and porcine TPO inhibition data. Microsomes were isolated from both rat and pig thyroid glands, and the guaiacol oxidation assay was performed for a training set of 12 chemicals, including previously reported TPO inhibitors, thyroid-disrupting chemicals thought to perturb other targets, and several previously untested chemicals, to determine the relative TPO inhibition responses across species. Concentration-response curves were derived for methimazole (MMI), dibutylphthalate (DBP), diethylhexylphthalate (DEHP), diethylphthalate (DEP), 3,5-dimethylpyrazole-1-methanol (DPM), iopanoic acid (IA), 2-mercaptobenzothiazole (MBT), sodium perchlorate (PERC), p-nonylphenol (PNP), 4-propoxyphenol (4POP), 6-propylthiouracil (PTU), and triclosan (TCS). MMI, PTU, MBT, DPM, 4POP, and at extremely high concentrations, PERC, inhibited TPO activity. Results demonstrated a strong qualitative concordance of response between the two species. All chemicals that inhibited TPO in porcine microsomes also inhibited TPO in rat microsomes. Hill model-derived IC50 values revealed approximate 1.5-to 50-fold differences in relative potency to MMI between species for positive chemicals. DPM, MBT, 4POP, and PTU exhibited greater relative potency to MMI using rat TPO versus porcine TPO, but rank order potency for inhibition was similar for the other test chemicals, with: PTU >MBT> DPM > 4POP > PERC for rat TPO and MBT> PTU> DPM > 4POP >PERC for porcine TPO. These data support the extrapolation of porcine TPO data to potential thyroid-disrupting activity in rodent models to evaluate TPO-inhibiting chemicals. Published by Elsevier Ireland Ltd. C1 [Paul, Katie B.] Oak Ridge Inst Sci & Educ, Oak Ridge, TN USA. [Paul, Katie B.; Hedge, Joan M.; Simmons, Steven O.] US EPA, Integrated Syst Toxicol Div, Natl Hlth & Environm Effects Res Lab, Off Res & Dev, Res Triangle Pk, NC 27711 USA. [Macherla, Chitralekha; Burgess, Emily; Hornung, Michael W.] US EPA, Midcontinent Ecol Div, Natl Hlth & Environm Effects Res Lab, Off Res & Dev, Duluth, MN 55804 USA. [Filer, Dayne L.; Crofton, Kevin M.] US EPA, Natl Ctr Computat Toxicol, Off Res & Dev, Res Triangle Pk, NC 27711 USA. RP Hornung, MW (reprint author), US EPA, Environm Effects Res Lab, Midcontinent Ecol Div, ORD, 6201 Congdon Blvd, Duluth, MN 55804 USA. EM Hornung.Michael@epa.gov RI Crofton, Kevin/J-4798-2015; OI Crofton, Kevin/0000-0003-1749-9971; Simmons, Steven/0000-0001-9079-1069 FU Oak Ridge Institute for Science and Education FX The authors would like to thank Kateland Antonazzo for technical assistance in necropsy and preparation of rat thyroid microsomes; Erica Nevalainen for technical assistance with the pTPO guaiacol oxidation assay; Dr. Matthew T. Martin for biostatistical consultation; Dr. Mary Gilbert for informative scientific discussion on thyroid biology and diet; and, John Havel for graphic design support. The authors would also like to thank Drs. Keith Houck and William Mundy for review of previous versions of this manuscript. K.B. Paul and D.L. Filer were supported by fellowships from the Oak Ridge Institute for Science and Education during this work. NR 90 TC 12 Z9 12 U1 6 U2 25 PU ELSEVIER IRELAND LTD PI CLARE PA ELSEVIER HOUSE, BROOKVALE PLAZA, EAST PARK SHANNON, CO, CLARE, 00000, IRELAND SN 0300-483X J9 TOXICOLOGY JI Toxicology PD OCT 4 PY 2013 VL 312 BP 97 EP 107 DI 10.1016/j.tox.2013.08.006 PG 11 WC Pharmacology & Pharmacy; Toxicology SC Pharmacology & Pharmacy; Toxicology GA 252LD UT WOS:000327005300012 PM 23959146 ER PT J AU Li, YZ Kessler, MR AF Li, Yuzhan Kessler, Michael R. TI Liquid crystalline epoxy resin based on biphenyl mesogen: Effect of magnetic field orientation during cure SO POLYMER LA English DT Article DE Liquid crystalline epoxy resins (LCERs); Magnetic field orientation; Thermomechanical properties ID AC ELECTRIC-FIELDS; RIGID-ROD; MECHANICAL-PROPERTIES; CURING KINETICS; POLYMER-FILMS; THERMOSETS; NETWORKS; PHOTOPOLYMERIZATION; POLYDOMAIN; MONOMERS AB A biphenyl based epoxy monomer, 4,4'-diglycidyloxybiphenyl (BP), was synthesized and cured with a tetra-functional amine, sulfanilamide (SAA), to obtain a liquid crystalline epoxy network. The curing behavior of BP with SAA was studied using differential scanning calorimetry, polarized optical microscopy, and parallel plate rheology. Macroscopic orientation of the liquid crystalline epoxy resins (LCERs) was achieved by curing in a high strength magnetic field, and quantified by an orientation parameter determined with wide angle X-ray diffraction. The effects of orientation on the glass transition temperature, coefficient of thermal expansion, and dynamic mechanical properties of the LCERs were investigated. The results reveal that the formation of the liquid crystalline phase has a dramatic influence on the curing reaction, leading to a decrease in viscosity of the reacting system. Oriented LCERs exhibit anisotropic thermal expansion behavior and significant improvements of thermomechanical properties. (C) 2013 Elsevier Ltd. All rights reserved. C1 [Li, Yuzhan; Kessler, Michael R.] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA USA. [Kessler, Michael R.] US DOE, Ames Lab, Ames, IA 50011 USA. [Li, Yuzhan; Kessler, Michael R.] Washington State Univ, Sch Mech & Mat Engn, Pullman, WA 99164 USA. RP Kessler, MR (reprint author), Washington State Univ, Sch Mech & Mat Engn, POB 642920, Pullman, WA 99164 USA. EM MichaelR.Kessler@wsu.edu RI Kessler, Michael/C-3153-2008 OI Kessler, Michael/0000-0001-8436-3447 FU Air Force Office of Scientific Research (AFOSR) [FA9550-12-1-0108] FX The authors would like to thank Dr. Scott Schlorholtz in the Materials Analysis Research Laboratory at Iowa State University for his help in X-ray diffraction tests. Support from the Air Force Office of Scientific Research (AFOSR) Award No. FA9550-12-1-0108 is gratefully acknowledged. NR 34 TC 7 Z9 7 U1 2 U2 41 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0032-3861 EI 1873-2291 J9 POLYMER JI Polymer PD OCT 4 PY 2013 VL 54 IS 21 BP 5741 EP 5746 DI 10.1016/j.polymer.2013.08.005 PG 6 WC Polymer Science SC Polymer Science GA 241YI UT WOS:000326204200036 ER PT J AU Munshi, P Stanley, CB Ghimire-Rijal, S Lu, X Myles, DA Cuneo, MJ AF Munshi, Parthapratim Stanley, Christopher B. Ghimire-Rijal, Sudipa Lu, Xun Myles, Dean A. Cuneo, Matthew J. TI Molecular details of ligand selectivity determinants in a promiscuous beta-glucan periplasmic binding protein SO BMC STRUCTURAL BIOLOGY LA English DT Article DE Periplasmic binding protein; Carbohydrate recognition; Laminarin; ABC transport; Ligand specificity ID CONFORMATIONAL-CHANGES; ESCHERICHIA-COLI; ANGSTROM RESOLUTION; CRYSTAL-STRUCTURE; THERMOTOGA-MARITIMA; ACID-BINDING; D-ALLOSE; TRANSPORT; MALTOSE; RECEPTOR AB Background: Members of the periplasmic binding protein (PBP) superfamily utilize a highly conserved inter-domain ligand binding site that adapts to specifically bind a chemically diverse range of ligands. This paradigm of PBP ligand binding specificity was recently altered when the structure of the Thermotoga maritima cellobiose-binding protein (tmCBP) was solved. The tmCBP binding site is bipartite, comprising a canonical solvent-excluded region (subsite one), adjacent to a solvent-filled cavity (subsite two) where specific and semi-specific ligand recognition occur, respectively. Results: A molecular level understanding of binding pocket adaptation mechanisms that simultaneously allow both ligand specificity at subsite one and promiscuity at subsite two has potentially important implications in ligand binding and drug design studies. We sought to investigate the determinants of ligand binding selectivity in tmCBP through biophysical characterization of tmCBP in the presence of varying beta-glucan oligosaccharides. Crystal structures show that whilst the amino acids that comprise both the tmCBP subsite one and subsite two binding sites remain fixed in conformation regardless of which ligands are present, the rich hydrogen bonding potential of water molecules may facilitate the ordering and the plasticity of this unique PBP binding site. Conclusions: The identification of the roles these water molecules play in ligand recognition suggests potential mechanisms that can be utilized to adapt a single ligand binding site to recognize multiple distinct ligands. C1 [Munshi, Parthapratim; Stanley, Christopher B.; Ghimire-Rijal, Sudipa; Lu, Xun; Myles, Dean A.; Cuneo, Matthew J.] Oak Ridge Natl Lab, Neutron Sci Directorate, Oak Ridge, TN 37831 USA. [Munshi, Parthapratim] Middle Tennessee State Univ, Dept Chem, Murfreesboro, TN 37132 USA. RP Cuneo, MJ (reprint author), Oak Ridge Natl Lab, Neutron Sci Directorate, Oak Ridge, TN 37831 USA. EM cuneomj@ornl.gov RI myles, dean/D-5860-2016; OI myles, dean/0000-0002-7693-4964; Cuneo, Matthew/0000-0002-1475-6656 FU U.S. Department of Energy, Office of Basic Energy Sciences; National Science Foundation [0922719] FX A portion of this research was performed at Oak Ridge National Laboratory's Spallation Neutron Source, sponsored by the U.S. Department of Energy, Office of Basic Energy Sciences. PM was funded in part through a research grant from the National Science Foundation (Award 0922719). NR 52 TC 2 Z9 2 U1 0 U2 11 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1472-6807 J9 BMC STRUCT BIOL JI BMC Struct. Biol. PD OCT 4 PY 2013 VL 13 AR 18 DI 10.1186/1472-6807-13-18 PG 11 WC Biophysics SC Biophysics GA 243TV UT WOS:000326341600001 PM 24090243 ER PT J AU Sahu, SN Anriany, Y Grim, CJ Kim, S Chang, Z Joseph, SW Cinar, HN AF Sahu, Surasri N. Anriany, Yuda Grim, Christopher J. Kim, Sungji Chang, Zenas Joseph, Sam W. Cinar, Hediye N. TI Identification of Virulence Properties in Salmonella Typhimurium DT104 Using Caenorhabditis elegans SO PLOS ONE LA English DT Article ID ENTERICA SEROVAR TYPHIMURIUM; MULTIDRUG-RESISTANCE REGION; UNFOLDED PROTEIN RESPONSE; INNATE IMMUNE-RESPONSE; C-ELEGANS; ANTIMICROBIAL PEPTIDES; MODEL HOST; INTESTINE; PATHOGEN; PATHWAY AB Salmonella enterica serover Typhimurium definitive phage type DT104, resistant to multiple antibiotics, is one of the most widespread Salmonella species in human infection worldwide. Although several cohort studies indicate that DT104 carrying the multidrug resistance (MDR) locus on salmonella genomic island 1 is a possible hyper-virulent strain compared to DT104 strains without MDR, or other Salmonella enterica serotypes, existing experimental evidence regarding virulence properties associated with the MDR region is controversial. To address this question, we constructed an isogenic MDR deletion (Delta MDR) mutant strain of DT104, SNS12, by allelic exchange and used Caenorhabditis elegans as a host model to assess differences in virulence between these two strains. SNS12 exhibited decreased virulence in C. elegans, and we observed increased colonization and proliferation of the intestine of C. elegans by DT104. The immune response against MDR-carrying DT104 appears to function through a non-canonical Unfolded Protein Response (UPR) pathway, namely prion-like-(QN-rich)-domain-bearing protein pathway (PQN), in a ced-1 dependent manner in C. elegans. Further, we also demonstrate that genes of the PQN pathway and antimicrobial peptide gene abf-2, are expressed at higher transcriptional levels in worms immediately following exposure to DT104, in comparison with worms exposed to SNS12. Altogether, our results suggest that the MDR region of Salmonella Typhimurium DT104 has a direct role in virulence against Caenorhabditis elegans. C1 [Sahu, Surasri N.; Grim, Christopher J.; Cinar, Hediye N.] US FDA, Div Virulence Assessment, Laurel, MD USA. [Sahu, Surasri N.; Grim, Christopher J.] Oak Ridge Inst Sci & Educ, Oak Ridge, TN USA. [Anriany, Yuda] Prince Georges Community Coll, Dept Biol Sci, Laurel, MD USA. [Kim, Sungji; Joseph, Sam W.] Kyungpook Natl Univ KNU, Taegu, South Korea. [Chang, Zenas] Univ Maryland, Dept Cell Biol & Mol Genet, College Pk, MD 20742 USA. RP Sahu, SN (reprint author), US FDA, Div Virulence Assessment, Laurel, MD USA. EM surasri.sahu@fda.hhs.gov FU Food and Drug Administration FX This study was funded by Food and Drug Administration intramural funding. The funder had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 44 TC 3 Z9 6 U1 1 U2 9 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD OCT 4 PY 2013 VL 8 IS 10 AR e76673 DI 10.1371/journal.pone.0076673 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 232JF UT WOS:000325489100144 PM 24124587 ER PT J AU Stetcu, I Talou, P Kawano, T Jandel, M AF Stetcu, I. Talou, P. Kawano, T. Jandel, M. TI Isomer production ratios and the angular momentum distribution of fission fragments SO PHYSICAL REVIEW C LA English DT Article ID THERMAL-NEUTRON FISSION; CROSS-SECTION RATIOS; PROMPT GAMMA RAYS; INDEPENDENT YIELDS; NUCLEAR-REACTIONS; CAPTURE; PU-239; U-233; ISOTOPES; FORMULA AB Latest generation fission experiments provide an excellent testing ground for theoretical models. In this contribution we compare the measurements for U-235(n(th),f), obtained with the Detector for Advanced Neutron Capture Experiments (DANCE) calorimeter at Los Alamos Neutron Science Center (LANSCE), with our full-scale simulation of the primary fragment de-excitation, using the recently developed CGMF code, based on a Monte Carlo implementation of the Hauser-Feshbach theoretical model. We compute the isomer ratios as a function of the initial angular momentum of the fission fragments, for which no direct information exists. Comparison with the available experimental data allows us to determine the initial spin distribution. We also study the dependence of the isomer ratio on the knowledge of the low-lying discrete spectrum input for nuclear fission reactions, finding a high degree of sensitivity. Finally, in the same Hauser-Feshbach approach, we calculate the isomer production ratio for thermal neutron capture on stable isotopes, where the initial conditions (spin, excitation energy, etc.) are well understood. We find that with the current parameters involved in Hauser-Feshbach calculations, we obtain up to a factor of 2 deviation from the measured isomer ratios. C1 [Stetcu, I.; Talou, P.; Kawano, T.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Jandel, M.] Los Alamos Natl Lab, C NR, Los Alamos, NM 87545 USA. RP Stetcu, I (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. NR 39 TC 8 Z9 8 U1 0 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0556-2813 EI 1089-490X J9 PHYS REV C JI Phys. Rev. C PD OCT 4 PY 2013 VL 88 IS 4 AR 044603 DI 10.1103/PhysRevC.88.044603 PG 8 WC Physics, Nuclear SC Physics GA 233LS UT WOS:000325570700001 ER PT J AU Cao, BF Veith, GM Diaz, RE Liu, J Stach, EA Adzic, RR Khalifah, PG AF Cao, Bingfei Veith, Gabriel M. Diaz, Rosa E. Liu, Jue Stach, Eric A. Adzic, Radoslav R. Khalifah, Peter G. TI Cobalt Molybdenum Oxynitrides: Synthesis, Structural Characterization, and Catalytic Activity for the Oxygen Reduction Reaction SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE electrochemistry; heterogeneous catalysis; nanoparticles; oxygen reduction; oxynitrides ID FUEL-CELL; ELECTROCATALYSTS; CATHODE; NITRIDES C1 [Cao, Bingfei; Liu, Jue; Khalifah, Peter G.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Veith, Gabriel M.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Diaz, Rosa E.; Stach, Eric A.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11793 USA. [Adzic, Radoslav R.; Khalifah, Peter G.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11793 USA. RP Khalifah, PG (reprint author), SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. EM kpete@bnl.gov RI Stach, Eric/D-8545-2011; LIU, JUE/J-6463-2014; LIU, JUE/I-8631-2016 OI Stach, Eric/0000-0002-3366-2153; LIU, JUE/0000-0003-1834-0356; LIU, JUE/0000-0002-4453-910X FU U.S. Department of Energy [DEAC02-98CH10886]; BNL LDRD [10-0012]; American Chemical Society Petroleum Research Fund; U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division FX This work was carried out at BNL under Contract DEAC02-98CH10886 with the U.S. Department of Energy, both in the Chemistry Department and in the Center for Functional Nanomaterials user facility. Primary funding was provided by BNL LDRD 10-0012 (P. G. K., R. R. A.). Acknowledgement is made to the Donors of the American Chemical Society Petroleum Research Fund for partial support of this research (P. G. K.). Research was partially supported by the U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division (GMV). We thank Nebojsa Marinkovic and Syed Khalid for on-site assistance in using X19A beamline at National Synchrotron Light Source, Brookhaven National Laboratory. NR 19 TC 37 Z9 37 U1 10 U2 150 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD OCT 4 PY 2013 VL 52 IS 41 BP 10753 EP 10757 DI 10.1002/anie.201303197 PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA 228AQ UT WOS:000325157600015 PM 24038934 ER PT J AU Lopez-Encarnacion, JM Tanabe, KK Johnson, MJA Jellinek, J AF Lopez-Encarnacion, Juan M. Tanabe, Kristine K. Johnson, Marc J. A. Jellinek, Julius TI Characterizing Metal Coordination Environments in Porous Organic Polymers: A Joint Density Functional Theory and Experimental Infrared Spectroscopy Study SO CHEMISTRY-A EUROPEAN JOURNAL LA English DT Article DE density functional calculations; IR spectroscopy; polymers; tantalum; transition metals ID CATALYTIC HYDROAMINOALKYLATION; UNACTIVATED OLEFINS; IMIDO COMPLEXES; HYDROAMINATION; METATHESIS; MOLECULES; NETWORKS; ALKANES; ALKYNES; SOLIDS C1 [Lopez-Encarnacion, Juan M.; Tanabe, Kristine K.; Johnson, Marc J. A.; Jellinek, Julius] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60349 USA. RP Johnson, MJA (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60349 USA. EM mjjohnson@anl.gov; jellinek@anl.gov FU Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences, US. Department of Energy [DE-AC02-06CH11357] FX This work was supported by the Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences, US. Department of Energy under Contract No. DE-AC02-06CH11357. J.M.L.E. wishes to thank Dr. M. Kryvohuz for fruitful discussions. NR 49 TC 2 Z9 2 U1 5 U2 31 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 0947-6539 J9 CHEM-EUR J JI Chem.-Eur. J. PD OCT 4 PY 2013 VL 19 IS 41 BP 13646 EP 13651 DI 10.1002/chem.201302812 PG 6 WC Chemistry, Multidisciplinary SC Chemistry GA 227SW UT WOS:000325135800008 PM 24092536 ER PT J AU Ma, J Dela Cruz, CD Hong, T Tian, W Aczel, AA Chi, SX Yan, JQ Dun, ZL Zhou, HD Matsuda, M AF Ma, J. Dela Cruz, C. D. Hong, Tao Tian, W. Aczel, A. A. Chi, Songxue Yan, J. -Q. Dun, Z. L. Zhou, H. D. Matsuda, M. TI Magnetic phase transition in the low-dimensional compound BaMn2Si2O7 SO PHYSICAL REVIEW B LA English DT Article ID QUANTUM SPIN CHAINS; ANTIFERROMAGNET; TEMPERATURE; BACO2SI2O7; OXIDES AB The structural and magnetic properties of BaMn2Si2O7 have been investigated. The magnetic susceptibility and specific heat, measured using single crystals, suggest that the quasi-one-dimensional magnetism originating from the loosely coupled Mn2+ chain carrying S = 5/2 is present at high temperatures, which is similar to the other quasi-one-dimensional barium silicates, BaM2Si2O7 (M: Cu and Co). The Neel temperature (T-N similar to 26 K) is high compared to the magnetic interaction along the chain (J = -6 K). Neutron powder diffraction study has revealed that the magnetic structure is long ranged with antiferromagnetic arrangement along the chain (c) direction and ferromagnetic arrangement along the a and b axes. Detailed structural analysis suggests that the interchain interaction via Mn-O-Mn bond along the a axis is relatively large, which makes the system behave more two-dimensionally in the ac plane and enhances T-N. C1 [Ma, J.; Dela Cruz, C. D.; Hong, Tao; Tian, W.; Aczel, A. A.; Chi, Songxue; Matsuda, M.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Yan, J. -Q.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Yan, J. -Q.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Dun, Z. L.; Zhou, H. D.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. RP Ma, J (reprint author), Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. RI Hong, Tao/F-8166-2010; Ma, Jie/C-1637-2013; Chi, Songxue/A-6713-2013; Aczel, Adam/A-6247-2016; Matsuda, Masaaki/A-6902-2016; Dun, Zhiling/F-5617-2016; dela Cruz, Clarina/C-2747-2013; Zhou, Haidong/O-4373-2016; Tian, Wei/C-8604-2013 OI Hong, Tao/0000-0002-0161-8588; Chi, Songxue/0000-0002-3851-9153; Aczel, Adam/0000-0003-1964-1943; Matsuda, Masaaki/0000-0003-2209-9526; Dun, Zhiling/0000-0001-6653-3051; dela Cruz, Clarina/0000-0003-4233-2145; Tian, Wei/0000-0001-7735-3187 FU Scientific User Facilities Division; Materials Sciences and Engineering Division, Office of Basic Energy Sciences, US Department of Energy FX The research at Oak Ridge National Laboratory was sponsored by the Scientific User Facilities Division (J.M., M. M., C. D. D. C., T. H., W. T., A. A. A., S. X. C.) and Materials Sciences and Engineering Division (J.Q.Y.), Office of Basic Energy Sciences, US Department of Energy. NR 26 TC 2 Z9 2 U1 0 U2 32 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD OCT 4 PY 2013 VL 88 IS 14 AR 144405 DI 10.1103/PhysRevB.88.144405 PG 8 WC Physics, Condensed Matter SC Physics GA 232ML UT WOS:000325497900003 ER PT J AU Lebedev, V Nagaitsev, S AF Lebedev, Valeri Nagaitsev, Sergei TI Comment on "Beamstrahlung considerations in laser-plasma-accelerator-based linear colliders" SO PHYSICAL REVIEW SPECIAL TOPICS-ACCELERATORS AND BEAMS LA English DT Editorial Material AB Schroeder, Esarey, Geddes, Benedetti, and Leemans [Phys. Rev. ST Accel. Beams 13, 101301 (2010) and Phys. Rev. ST Accel. Beams 15, 051301 (2012)] have proposed a set of parameters for a TeV-scale collider based on plasma wakefield accelerator principles. In particular, it is sugested that the luminosities greater than 10(34) cm(-2) s(-1) are attainable for an electron-positron collider. In this Comment we dispute this set of parameters on the basis of first principles. The interactions of accelerating beam with plasma impose fundamental limitations on beam properties and, thus, on attainable luminosity values. C1 [Lebedev, Valeri; Nagaitsev, Sergei] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. RP Lebedev, V (reprint author), Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. NR 4 TC 2 Z9 2 U1 0 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-4402 J9 PHYS REV SPEC TOP-AC JI Phys. Rev. Spec. Top.-Accel. Beams PD OCT 4 PY 2013 VL 16 IS 10 AR 108001 DI 10.1103/PhysRevSTAB.16.108001 PG 3 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA 230QW UT WOS:000325358300001 ER PT J AU Schroeder, CB Esarey, E Leemans, WP AF Schroeder, C. B. Esarey, E. Leemans, W. P. TI Reply to "Comment on 'Beamstrahlung considerations in laser-plasma-accelerator-based linear colliders' " SO PHYSICAL REVIEW SPECIAL TOPICS-ACCELERATORS AND BEAMS LA English DT Editorial Material ID CHANNEL AB We reply to Lebedev and Nagaitsev's foregoing Comment [Phys. Rev. ST Accel. Beams 16, 108001 (2013)]. We disagree with the conclusion of the Comment that scattering imposes a fundamental limitation on plasma-based accelerator technology. Laser-plasma accelerators are compatible with high-luminosity collider concepts. C1 [Schroeder, C. B.; Esarey, E.; Leemans, W. P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Schroeder, CB (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. OI Schroeder, Carl/0000-0002-9610-0166 NR 10 TC 1 Z9 1 U1 0 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1098-4402 J9 PHYS REV SPEC TOP-AC JI Phys. Rev. Spec. Top.-Accel. Beams PD OCT 4 PY 2013 VL 16 IS 10 AR 108002 DI 10.1103/PhysRevSTAB.16.108002 PG 2 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA 230QW UT WOS:000325358300002 ER EF