FN Thomson Reuters Web of Science™ VR 1.0 PT S AU Banks, JW Hittinger, JAF Connors, JM Woodward, CS AF Banks, J. W. Hittinger, J. A. F. Connors, J. M. Woodward, C. S. BE Li, J Yang, HT Machorro, E TI A posteriori error estimation via nonlinear error transport with application to shallow water SO RECENT ADVANCES IN SCIENTIFIC COMPUTING AND APPLICATIONS SE Contemporary Mathematics LA English DT Proceedings Paper CT 8th International Conference on Scientific Computing and Applications CY APR 01-04, 2012 CL Univ Nevada, Las Vegas, NV SP UNLV, Dept Math Sci HO Univ Nevada DE A posteriori error estimation; hyperbolic equations; finite volume methods; finite difference methods; weak solutions ID OVERLAPPING GRIDS; EQUATIONS; MESHES AB Numerical error estimation for time dependent hyperbolic problems is challenging for theoretical and practical reasons. In these systems, error can propagate long distances and produce effects far from the point of generation. In addition, nonlinear interactions of error, as well as discretization nonlinearities can play important roles and must be addressed. In this work, we investigate the use of error transport equations for a posteriori error estimation. We discuss the inclusion of nonlinearities in the error equations, which are particularly important for situations where local errors become large, such as near shocks. C1 [Banks, J. W.; Hittinger, J. A. F.; Connors, J. M.; Woodward, C. S.] Lawrence Livermore Natl Lab, Ctr Appl Sci Comp, Livermore, CA 94551 USA. RP Banks, JW (reprint author), Lawrence Livermore Natl Lab, Ctr Appl Sci Comp, Livermore, CA 94551 USA. EM banks20@llnl.gov RI Banks, Jeffrey/A-9718-2012; Woodward, Carol/M-4008-2014 NR 15 TC 0 Z9 0 U1 0 U2 4 PU AMER MATHEMATICAL SOC PI PROVIDENCE PA P.O. BOX 6248, PROVIDENCE, RI 02940 USA SN 0271-4132 BN 978-0-8218-8737-0 J9 CONTEMP MATH PY 2013 VL 586 BP 35 EP 42 DI 10.1090/conm/586/11646 PG 8 WC Mathematics SC Mathematics GA BFD22 UT WOS:000319240200004 ER PT J AU Piwowar, AM Keskin, S Delgado, MO Shen, K Hue, JJ Lanekoff, I Ewing, AG Winograd, N AF Piwowar, Alan M. Keskin, Selda Delgado, Melissa Ortiz Shen, Kan Hue, Jonathan J. Lanekoff, Ingela Ewing, Andrew G. Winograd, Nicholas TI C60-ToF SIMS imaging of frozen hydrated HeLa cells SO SURFACE AND INTERFACE ANALYSIS LA English DT Article; Proceedings Paper CT 18th International Conferenceon Secondary Ion Mass Spectrometry (SIMS XVIII) CY SEP 18-23, 2011 CL Trento, ITALY DE C60; HeLa cell; frozen-hydrated; sample preparation; biological imaging ID ION MASS-SPECTROMETRY; TOF-SIMS AB Sample preparation continues to be a major challenge for SIMS studies of biological materials. Maintaining the native hydrated state of the material is important for preserving both chemical and spatial information. Here, we discuss a method that combines a sample wash and dry protocol followed by plunge-freezing in liquid ethane for a frozen-hydrated analysis of mammalian cells (HeLa). This method allows for the removal of the growth medium and maintains the hydrated state of the cells so that they can be prepared frozen-hydrated without the need for a freeze-fracture device. The cells, which were grown on silicon, were successfully regrown after the cleaning procedure, confirming that a significant portion of the cells remain undamaged during the wash and dry procedure. Results from preliminary SIMS measurements show that is it possible to detect a large variety of biomolecular signals, including intact lipids from the plasma membrane in the mass range of 700-900 Da from single cells, with little external water interference at the surface. Copyright (C) 2012 John Wiley & Sons, Ltd. C1 [Piwowar, Alan M.] Dow Chem Co USA, Spring House, PA 19002 USA. [Piwowar, Alan M.; Keskin, Selda; Delgado, Melissa Ortiz; Shen, Kan; Hue, Jonathan J.; Winograd, Nicholas] Penn State Univ, Dept Chem, University Pk, PA 16802 USA. [Lanekoff, Ingela] Pacific NW Natl Lab, Richland, WA 99352 USA. [Ewing, Andrew G.] Univ Gothenburg, Dept Chem, SE-41296 Gothenburg, Sweden. RP Piwowar, AM (reprint author), Dow Chem Co USA, 727 Norristown Rd, Spring House, PA 19002 USA. EM AMPiwowar@dow.com OI Winograd, Nicholas/0000-0002-2690-7714 FU National Institutes of Health LIPID MAPS consortium [GM 069338-07]; [2R01 EB002016-18] FX The authors acknowledge the National Institutes of Health LIPID MAPS consortium (GM 069338-07) and grant 2R01 EB002016-18 for partial financial support, and extend a special thanks to Irene Lee of Case Western Reserve University for her help with HeLa cell preparation. NR 11 TC 20 Z9 20 U1 3 U2 35 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0142-2421 EI 1096-9918 J9 SURF INTERFACE ANAL JI Surf. Interface Anal. PD JAN PY 2013 VL 45 IS 1 SI SI BP 302 EP 304 DI 10.1002/sia.4882 PG 3 WC Chemistry, Physical SC Chemistry GA 145WB UT WOS:000319048700077 PM 23585702 ER PT J AU Ohlhausen, JA Coker, EN Ambrosini, A Miller, JE AF Ohlhausen, James A. (Tony) Coker, Eric N. Ambrosini, Andrea Miller, James E. TI ToF-SIMS analysis of iron oxide particle oxidation by isotopic and multivariate analysis SO SURFACE AND INTERFACE ANALYSIS LA English DT Article; Proceedings Paper CT 18th International Conferenceon Secondary Ion Mass Spectrometry (SIMS XVIII) CY SEP 18-23, 2011 CL Trento, ITALY DE ToF-SIMS; multivariate analysis; isotopic analysis; oxidation; reduction; YSZ; yttria stabilized zirconia; iron oxide ID ION MASS-SPECTROMETRY; STATISTICAL-ANALYSIS; IMAGES AB A procedure for quantitative time-of-flight secondary ion mass spectrometry (ToF-SIMS) analysis of the re-oxidation thermally-reduced of iron oxide particles in a ceramic matrix is discussed. Iron oxide is reacted with yttria stabilized zirconia (YSZ) to create a composite that facilitates the high-temperature reduction of CO2 and H2O to produce CO and H-2 (syngas). The reactivity of this two-step solar-thermochemical process is being investigated by varying the concentration of iron in YSZ up to and past its solid solubility point, thus affecting the size of iron oxide particles in the matrix, and hence their rate and extent of re-oxidation. YSZ samples containing natural abundance iron oxide were mixed with an organic binder, isostatically pressed into a disc and calcined in air at 1450 degrees C. The discs (similar to 10mm diameter, 2mm thickness) were thermally reduced in inert gas at 1400 degrees C and then re-oxidized at 1100 degrees C in the presence of (CO2)-O-18. The ratio of O-18 to O-16 shows the extent of oxygen exchange for each iron oxide particle. ToF-SIMS data are acquired in a fashion that maximizes the ability to correct for detector saturation, thus providing quantitative oxygen isotopic results with little error. The data analysis method uses a combination of multivariate analysis for particle identification and conventional analysis for quantitative isotopic ratioing. The results indicate that large iron oxide particles are only poorly utilized, likely due to slow transport, as O-18 penetration into the particles is limited. Published 2012. This article is a U.S. Government work and is in the public domain in the USA. C1 [Ohlhausen, James A. (Tony); Coker, Eric N.; Ambrosini, Andrea; Miller, James E.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Ohlhausen, JA (reprint author), Sandia Natl Labs, POB 5800,MS 0886, Albuquerque, NM 87185 USA. EM jaohlha@sandia.gov RI Miller, James/C-1128-2011 OI Miller, James/0000-0001-6811-6948 FU Laboratory Directed Research and Development program at Sandia National Laboratories; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported by the Laboratory Directed Research and Development program at Sandia National Laboratories, in the form of a Grand Challenge project entitled 'Reimagining Liquid Transportation Fuels: Sunshine to Petrol.' Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 7 TC 1 Z9 1 U1 1 U2 11 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0142-2421 EI 1096-9918 J9 SURF INTERFACE ANAL JI Surf. Interface Anal. PD JAN PY 2013 VL 45 IS 1 SI SI BP 320 EP 323 DI 10.1002/sia.5140 PG 4 WC Chemistry, Physical SC Chemistry GA 145WB UT WOS:000319048700082 ER PT J AU Mudiyanselage, K Senanayake, SD Feria, L Kundu, S Baber, AE Graciani, J Vidal, AB Agnoli, S Evans, J Chang, R Axnanda, S Liu, Z Sanz, JF Liu, P Rodriguez, JA Stacchiola, DJ AF Mudiyanselage, Kumudu Senanayake, Sanjaya D. Feria, Leticia Kundu, Shankhamala Baber, Ashleigh E. Graciani, Jesus Vidal, Alba B. Agnoli, Stefano Evans, Jaime Chang, Rui Axnanda, Stephanus Liu, Zhi Sanz, Javier F. Liu, Ping Rodriguez, Jose A. Stacchiola, Dario J. TI Importance of the Metal-Oxide Interface in Catalysis: In Situ Studies of the Water-Gas Shift Reaction by Ambient-Pressure X-ray Photoelectron Spectroscopy SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE ceria; heterogeneous catalysis; nanocatalysis; surface chemistry; watergas shift reaction ID SURFACE-CHEMISTRY; MECHANISM; NANOPARTICLES; COPPER; CO2; PHOTOEMISSION; CEOX/CU(111); ADSORPTION; OXIDATION; AU(111) C1 [Mudiyanselage, Kumudu; Senanayake, Sanjaya D.; Kundu, Shankhamala; Baber, Ashleigh E.; Graciani, Jesus; Vidal, Alba B.; Agnoli, Stefano; Liu, Ping; Rodriguez, Jose A.; Stacchiola, Dario J.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Feria, Leticia; Graciani, Jesus; Sanz, Javier F.] Univ Seville, Dept Quim Fis, E-41012 Seville, Spain. [Evans, Jaime] Cent Univ Venezuela, Fac Ciencias, Caracas 1020A, Venezuela. [Chang, Rui] Shanghai Inst Microsyst & Informat Technol, Shanghai 200050, Peoples R China. [Axnanda, Stephanus; Liu, Zhi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Stacchiola, DJ (reprint author), Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. EM djs@bnl.gov RI Stacchiola, Dario/B-1918-2009; Axnanda, Stephanus/G-9236-2011; Kundu, Shankhamala/C-4875-2012; Liu, Zhi/B-3642-2009; Senanayake, Sanjaya/D-4769-2009; Mudiyanselage, Kumudu/B-2277-2013 OI Stacchiola, Dario/0000-0001-5494-3205; Liu, Zhi/0000-0002-8973-6561; Senanayake, Sanjaya/0000-0003-3991-4232; Mudiyanselage, Kumudu/0000-0002-3539-632X FU US DOE, Office of BES [DE-AC02-98CH10086]; Ministerio de Economia y Competitividad (Spain) [MAT2012-31526, CSD2008-0023]; INTEVEP; IDB FX Research carried at BNL was financed by the US DOE, Office of BES (Grant No. DE-AC02-98CH10086). Some of the calculations were performed at the Center for Functional Nanomaterials at BNL. The main theoretical part was carried out by the group of J.F.S. and funded by the Ministerio de Economia y Competitividad (Spain, grants MAT2012-31526 and CSD2008-0023). Computational resources were provided by the Barcelona Centro Nacional de Supercomputacion (Spain). J.E. thanks INTEVEP and IDB for grants used for the research in Venezuela. NR 36 TC 98 Z9 98 U1 29 U2 275 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PY 2013 VL 52 IS 19 BP 5101 EP 5105 DI 10.1002/anie.201210077 PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA 142LV UT WOS:000318799800019 PM 23576363 ER PT J AU Aydin, C Kulkarni, A Chi, MF Browning, ND Gates, BC AF Aydin, Ceren Kulkarni, Apoorva Chi, Miaofang Browning, Nigel D. Gates, Bruce C. TI Three-Dimensional Structural Analysis of MgO-Supported Osmium Clusters by Electron Microscopy with Single-Atom Sensitivity SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE clusters; electron microscopy; osmium; supported catalysts ID CARBONYL CLUSTERS; OXIDE SUPPORTS; COMPLEXES; CATALYSTS; NANOPARTICLES; MONONUCLEAR; OS3(CO)12; BEHAVIOR; LIGANDS; DIANION C1 [Aydin, Ceren; Kulkarni, Apoorva; Gates, Bruce C.] Univ Calif Davis, Dept Chem Engn & Mat Sci, Davis, CA 95616 USA. [Chi, Miaofang] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37830 USA. [Browning, Nigel D.] Pacific NW Natl Lab, Fundamental & Computat Sci Div, Richland, WA 99352 USA. RP Gates, BC (reprint author), Univ Calif Davis, Dept Chem Engn & Mat Sci, 1 Shields Ave, Davis, CA 95616 USA. EM bcgates@ucdavis.edu RI Chi, Miaofang/Q-2489-2015; OI Chi, Miaofang/0000-0003-0764-1567; Browning, Nigel/0000-0003-0491-251X FU Department of Energy (DOE) [DE-SC0005822, DE-FG02-03ER46057]; University of California Lab Fee Program; Division of Scientific User Facilities, DOE Office of Science, Basic Energy Sciences FX This work was supported by the Department of Energy (DOE), grants DE-SC0005822 and DE-FG02-03ER46057 (C. A.) and the University of California Lab Fee Program. The electron microscopy experiments were performed at the Oak Ridge National Laboratory Shared Research Equipment (ShaRE) User Facility, which is supported by the Division of Scientific User Facilities, DOE Office of Science, Basic Energy Sciences. We acknowledge beam time and support of the DOE Office of Science, Materials Sciences, for its role in the operation and development of beamlines 4-1 and 10-2 at the Stanford Synchrotron Radiation Lightsource. NR 32 TC 4 Z9 4 U1 6 U2 56 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PY 2013 VL 52 IS 20 BP 5262 EP 5265 DI 10.1002/anie.201300238 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA 136OC UT WOS:000318370200009 PM 23592186 ER PT J AU Kuepper, K Derks, C Taubitz, C Prinz, M Joly, L Kappler, JP Postnikov, A Yang, WL Kuznetsova, TV Wiedwald, U Ziemann, P Neumann, M AF Kuepper, Karsten Derks, Christine Taubitz, Christian Prinz, Manuel Joly, Loic Kappler, Jean-Paul Postnikov, Andrei Yang, Wanli Kuznetsova, Tatyana V. Wiedwald, Ulf Ziemann, Paul Neumann, Manfred TI Electronic structure and soft-X-ray-induced photoreduction studies of iron-based magnetic polyoxometalates of type {(M)M-5}(12)Fe-30(III) (M = Mo-VI, W-VI) SO DALTON TRANSACTIONS LA English DT Article ID EXCHANGE INTERACTIONS; MOLECULAR MAGNETS; GIANT CLUSTERS; SPECTROSCOPY; DICHROISM; CHEMISTRY; LINKING; PHOTOCHEMISTRY; ABSORPTION; LIGAND AB Giant Keplerate-type molecules with a {Mo72Fe30} core show a number of very interesting properties, making them particularly promising for various applications. So far, only limited data on the electronic structure of these molecules from X-ray spectra and electronic structure calculations have been available. Here we present a combined electronic and magnetic structure study of three Keplerate-type nanospheres-two with a {Mo72Fe30} core and one with a {W72Fe30} core by means of X-ray absorption spectroscopy, X-ray magnetic circular dichroism (XMCD), SQUID magnetometry, and complementary theoretical approaches. Furthermore, we present detailed studies of the Fe3+-to-Fe2+ photoreduction process, which is induced under soft X-ray radiation in these molecules. We observe that the photoreduction rate greatly depends on the ligand structure surrounding the Fe ions, with negatively charged ligands leading to a dramatically reduced photoreduction rate. This opens the possibility of tailoring such polyoxometalates by X-ray spectroscopic studies and also for potential applications in the field of X-ray induced photochemistry. C1 [Kuepper, Karsten; Wiedwald, Ulf; Ziemann, Paul] Univ Ulm, Inst Solid State Phys, D-89069 Ulm, Germany. [Kuepper, Karsten; Derks, Christine; Taubitz, Christian; Prinz, Manuel; Neumann, Manfred] Univ Osnabruck, Dept Phys, D-49069 Osnabruck, Germany. [Joly, Loic; Kappler, Jean-Paul] Univ Strasbourg, IPCMS UCMS CNRS 7504, F-67034 Strasbourg 2, France. [Postnikov, Andrei] Univ Lorraine, LCP A2MC, F-57078 Metz, France. [Postnikov, Andrei] Univ Bielefeld, Fac Phys, D-33501 Bielefeld, Germany. [Yang, Wanli] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Kuznetsova, Tatyana V.] Russian Acad Sci, Ural Div, Inst Met Phys, Ekaterinburg 620990, Russia. RP Kuepper, K (reprint author), Univ Ulm, Inst Solid State Phys, Albert Einstein Allee 11, D-89069 Ulm, Germany. EM kkuepper@uos.de RI Kuznetsova, Tatyana/J-4806-2013; Wiedwald, Ulf/E-4625-2011; Yang, Wanli/D-7183-2011; Kupper, Karsten/G-1397-2016; Joly, Loic/I-2391-2016 OI Kuznetsova, Tatyana/0000-0003-4302-9607; Yang, Wanli/0000-0003-0666-8063; Joly, Loic/0000-0002-0137-2821 FU BESSY II (Helmholtz - Zentrum Berlin), Germany [DE-AC02-05CH11231]; PhD programme of the Federal State of Lower Saxony, Germany; DFG [GRK 965, FOR 945]; EU; RFBR [11-02-01221, 11-02-00379]; bilateral Program "Russian-German Laboratory at BESSY"; [SFB 569] FX We are indebted to A. Muller and co-workers for generously providing samples. We thank J. Schnack for carefully reading our manuscript and suggesting very valuable improvements. This work was performed at the Advanced Light Source, Lawrence Berkeley National Laboratory, Berkeley, USA; which is operated under contract No. DE-AC02-05CH11231, BESSY II (Helmholtz - Zentrum Berlin), Germany, and the Swiss Light Source (Paul Scherrer Institute), Switzerland. Financial and travel support from the SFB 569, the PhD programme of the Federal State of Lower Saxony, Germany, the DFG GRK 965, the DFG FOR 945, and the EU's Seventh Framework Programme are gratefully acknowledged. We thank all beamline scientists for their excellent and generous technical support. T. V. K thanks the RFBR (Project Nos. 11-02-01221 and 11-02-00379) and bilateral Program "Russian-German Laboratory at BESSY" for financial support. NR 41 TC 8 Z9 8 U1 2 U2 35 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1477-9226 J9 DALTON T JI Dalton Trans. PY 2013 VL 42 IS 22 BP 7924 EP 7935 DI 10.1039/c3dt32759k PG 12 WC Chemistry, Inorganic & Nuclear SC Chemistry GA 144MK UT WOS:000318943400014 PM 23403844 ER PT J AU Xu, SL Feng, DH Yan, Z Zhang, L Li, NH Jing, L Wang, JH AF Xu, Shaolun Feng, Donghan Yan, Zheng Zhang, Liang Li, Naihu Jing, Lei Wang, Jianhui TI Ant-Based Swarm Algorithm for Charging Coordination of Electric Vehicles SO INTERNATIONAL JOURNAL OF DISTRIBUTED SENSOR NETWORKS LA English DT Article ID OPTIMIZATION AB Uncontrolled charging of large-scale electric vehicles (EVs) can affect the safe and economic operation of power systems, especially at the distribution level. The centralized EVs charging optimization methods require complete information of physical appliances and using habits, which will cause problems of high dimensionality and communication block. Given this, an ant-based swarm algorithm(ASA) is proposed to realize the EVs charging coordination at the transformer level, which can overcome the drawbacks of centralized control method. First, the EV charging load model is developed, and the charging management structure based on swarm intelligence is presented. Second, basic data of the EV using habit is sampled by the Monte Carlo method, and the ASA is applied to realize the load valley filling. The load fluctuation and the transformer capacity are also considered in the algorithm. Finally, the charging coordination of 500 EVs under a 12.47 KV transformer is simulated to demonstrate the validity of the proposed method. C1 [Xu, Shaolun; Feng, Donghan; Yan, Zheng; Zhang, Liang] Minist Educ, Key Lab Control Power Transmiss & Convers, Shanghai 200240, Peoples R China. [Li, Naihu; Jing, Lei] Alstom Grid Technol Ctr Co Ltd, Shanghai 200240, Peoples R China. [Wang, Jianhui] Argonne Natl Lab, Decis & Informat Sci Div, Argonne, IL 60439 USA. RP Feng, DH (reprint author), Minist Educ, Key Lab Control Power Transmiss & Convers, Shanghai 200240, Peoples R China. EM seed@sjtu.edu.cn RI Feng, Donghan/I-9213-2016; OI Feng, Donghan/0000-0002-9642-4777 FU National High-tech R&D (863) Program of China [2012AA050803]; National Natural Science Foundation of China [51007058]; Research Fund for the Doctoral Program of Higher Education of China [20120073110020]; SMC Excellent Young Faculty Program of Shanghai Jiao Tong University FX This work was supported by the National High-tech R&D (863) Program of China (Grant no. 2012AA050803), National Natural Science Foundation of China (Grant no. 51007058), Research Fund for the Doctoral Program (for Ph.D. Supervisor) of Higher Education of China (Grant no. 20120073110020), and SMC Excellent Young Faculty Program of Shanghai Jiao Tong University. NR 25 TC 3 Z9 3 U1 0 U2 17 PU SAGE PUBLICATIONS INC PI THOUSAND OAKS PA 2455 TELLER RD, THOUSAND OAKS, CA 91320 USA SN 1550-1477 J9 INT J DISTRIB SENS N JI Int. J. Distrib. Sens. Netw. PY 2013 AR 268942 DI 10.1155/2013/268942 PG 13 WC Computer Science, Information Systems; Telecommunications SC Computer Science; Telecommunications GA 147JX UT WOS:000319164100001 ER PT J AU Mingesz, R Kish, LB Gingl, Z Granqvist, CG Wen, H Peper, F Eubanks, T Schmera, G AF Mingesz, Robert Kish, Laszlo Bela Gingl, Zoltan Granqvist, Claes-Goran Wen, He Peper, Ferdinand Eubanks, Travis Schmera, Gabor TI UNCONDITIONAL SECURITY BY THE LAWS OF CLASSICAL PHYSICS SO METROLOGY AND MEASUREMENT SYSTEMS LA English DT Article DE information theoretic security; unconditional security; secure key exchange; secure key distribution; quantum encryption ID JOHNSON-LIKE NOISE; TAILORED BRIGHT ILLUMINATION; QUANTUM CRYPTOGRAPHY; THERMAL AGITATION; SYSTEM; ATTACK; STATES; SUPERPOSITION; CONDUCTORS; PROTOCOLS AB There is an ongoing debate about the fundamental security of existing quantum key exchange schemes. This debate indicates not only that there is a problem with security but also that the meanings of perfect, imperfect, conditional and unconditional (information theoretic) security in physically secure key exchange schemes are often misunderstood. It has been shown recently that the use of two pairs of resistors with enhanced Johnson-noise and a Kirchhoff-loop - i.e., a Kirchhoff-Law-Johnson-Noise (KLJN) protocol - for secure key distribution leads to information theoretic security levels superior to those of today's quantum key distribution. This issue is becoming particularly timely because of the recent full cracks of practical quantum communicators, as shown in numerous peer-reviewed publications. The KLJN system is briefly surveyed here with discussions about the essential questions such as (i) perfect and imperfect security characteristics of the key distribution, and (ii) how these two types of securities can be unconditional (or information theoretical). C1 [Mingesz, Robert; Gingl, Zoltan] Univ Szeged, Dept Tech Informat, H-6701 Szeged, Hungary. [Kish, Laszlo Bela; Wen, He] Texas A&M Univ, Dept Elect & Comp Engn, College Stn, TX 77843 USA. [Granqvist, Claes-Goran] Uppsala Univ, Dept Engn Sci, SE-75121 Uppsala, Sweden. [Wen, He] Hunan Univ, Coll Elect & Informat Engn, Changsha 410082, Hunan, Peoples R China. [Peper, Ferdinand] Natl Inst Informat & Commun Technol, Kobe, Hyogo 6512492, Japan. [Eubanks, Travis] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Schmera, Gabor] Space & Naval Warfare Syst Ctr, San Diego, CA 92152 USA. RP Kish, LB (reprint author), Texas A&M Univ, Dept Elect & Comp Engn, College Stn, TX 77843 USA. EM mingesz@inf.u-szeged.hu; Laszlo.Kish@ece.tamu.edu; Claes-Goran.Granqvist@Angstrom.uu.se; he_wen82@126.com; peper@nict.go.jp; tweuban@sandia.gov; gabe.schmera@navy.mil RI Gingl, Zoltan/E-8262-2011; Wen, He/F-9834-2010 OI Gingl, Zoltan/0000-0001-6570-2685; Wen, He/0000-0001-8024-1899 FU National Natural Science Foundation of China [61002035]; [TAMOP-4.2.1/B-09/1/KONV-2010-0005] FX LBK is grateful to Horace Yuen for discussions on fundamental problems of current QKD schemes, on his new improved scheme, and on the general requirements for physically secure key exchange. LBK is also indebted to Vincent Poor for a discussion on unconditional (information theoretic) security of practical secure physical systems with imperfect security. RM and ZG were partially supported by grant TAMOP-4.2.1/B-09/1/KONV-2010-0005. HW was partially supported by the National Natural Science Foundation of China under grant 61002035. NR 58 TC 19 Z9 19 U1 2 U2 12 PU POLISH ACAD SCIENCES COMMITTEE METROLOGY & RES EQUIPMENT PI WARSAW PA UL MIODOWA 10, WARSAW, 00251, POLAND SN 0860-8229 J9 METROL MEAS SYST JI Metrol. Meas. Syst. PY 2013 VL 20 IS 1 BP 3 EP 16 DI 10.2478/mms-2013-0001 PG 14 WC Instruments & Instrumentation SC Instruments & Instrumentation GA 143QM UT WOS:000318882300001 ER PT J AU Hsin, CL Wingert, M Huang, CW Guo, H Shih, TJ Suh, J Wang, K Wu, JQ Wu, WW Chen, RK AF Hsin, Cheng-Lun Wingert, Matthew Huang, Chun-Wei Guo, Hua Shih, Ten-Jen Suh, Joonki Wang, Kevin Wu, Junqiao Wu, Wen-Wei Chen, Renkun TI Phase transformation and thermoelectric properties of bismuth-telluride nanowires SO NANOSCALE LA English DT Article ID SILICON NANOWIRES; PERFORMANCE AB Thermoelectric materials have attracted much attention due to the current interest in energy conversion and recent advancements in nano-engineering. A simple approach to synthesize BiTe and Bi2Te3 micro/nanowires was developed by combining solution chemistry reactions and catalyst-free vapor-solid growth. A pathway to transform the as-grown BiTe nanostructures into Bi2Te3 can be identified through the Bi-Te phase diagram. Structural characterization of these products was identified using standard microscopy practices. Meanwhile, thermoelectric properties of individual Bi-Te compound micro/nanowires were determined by the suspended microdevice technique. This approach provides an applicable route to synthesize advanced high performance thermoelectric materials in quantities and can be used for a wide range of low-dimensional structures. C1 [Hsin, Cheng-Lun; Shih, Ten-Jen] Natl Cent Univ, Dept Elect Engn, Tao Yuan 32001, Taiwan. [Wingert, Matthew; Chen, Renkun] Univ Calif La Jolla, Dept Mech & Aerosp Engn, San Diego, CA 92093 USA. [Huang, Chun-Wei; Wu, Wen-Wei] Natl Chiao Tung Univ, Dept Mat Sci & Engn, Hsinchu 300, Taiwan. [Guo, Hua; Suh, Joonki; Wang, Kevin; Wu, Junqiao] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Wu, Junqiao] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Hsin, CL (reprint author), Natl Cent Univ, Dept Elect Engn, Tao Yuan 32001, Taiwan. EM clhsin@ee.ncu.edu.tw; rkchen@ucsd.edu RI Guo, Hua/D-5066-2013; Chen, Renkun/J-2400-2014 OI Chen, Renkun/0000-0001-7526-4981 FU Taiwan National Science Council (NSC) [101-2218-E-008-014-MY2, 101-3113-P-008-008-, 100-2628-E-009-023-MY3]; National Science Foundation (NSF) [CBET-0932905]; Department of Energy BES-LBL thermoelectrics program [DE-AC02-05-CH11231]; National Center for Electron Microscopy, Lawrence Berkeley Lab [DE-AC02-05CH11231] FX The authors acknowledge the support from Taiwan National Science Council (NSC) Grants 101-2218-E-008-014-MY2, 101-3113-P-008-008-, 100-2628-E-009-023-MY3, National Science Foundation (NSF) under Grant no. CBET-0932905, Department of Energy BES-LBL thermoelectrics program (DE-AC02-05-CH11231) and National Center for Electron Microscopy, Lawrence Berkeley Lab (DE-AC02-05CH11231). NR 27 TC 26 Z9 26 U1 7 U2 87 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2040-3364 J9 NANOSCALE JI Nanoscale PY 2013 VL 5 IS 11 BP 4669 EP 4672 DI 10.1039/c3nr00876b PG 4 WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 145IL UT WOS:000319008700010 PM 23619552 ER PT J AU Mao, YB Parsons, J McCloy, JS AF Mao, Yuanbing Parsons, Jason McCloy, John S. TI Magnetic properties of double perovskite La2BMnO6 (B = Ni or Co) nanoparticles SO NANOSCALE LA English DT Article ID SPIN-GLASS BEHAVIOR; LOW-TEMPERATURE SYNTHESIS; MOLTEN-SALT SYNTHESIS; ROOM-TEMPERATURE; LA2NIMNO6; LA2COMNO6; FILMS; LAALO3; SRTIO3 AB Double perovskite La2BMnO6 (B = Ni and Co) nanoparticles with average particle size of similar to 50 nm were synthesized using a facile, environmentally friendly, and scalable molten-salt reaction at 700 degrees C in air. Their structural and morphological properties were characterized by X-ray diffraction and transmission electron microscopy. Their magnetic properties were evaluated and compared using dc magnetic M-T and M-H, and ac magnetic susceptibility versus frequency, temperature, and field for the first time. The dc magnetization curves show paramagnetic-ferromagnetic transitions at T-C similar to 275 and 220 K for La2NiMnO6 (LNMO) and La2CoMnO6 (LCMO) nanoparticles, respectively. ac susceptibility revealed that the LCMO nanoparticles had a single magnetic transition indicative of Co2+-O2--Mn4+ ordering, whereas the LNMO nanoparticles showed more complex magnetic behaviors suggesting a re-entrant spin glass. C1 [Mao, Yuanbing; Parsons, Jason] Univ Texas Pan Amer, Dept Chem, Edinburg, TX 78539 USA. [McCloy, John S.] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. RP Mao, YB (reprint author), Univ Texas Pan Amer, Dept Chem, Edinburg, TX 78539 USA. EM maoy@utpa.edu; john.mccloy@pnnl.gov RI McCloy, John/D-3630-2013 OI McCloy, John/0000-0001-7476-7771 FU University of Texas-Pan American; National Science Foundation under DMR [0934157]; U.S. Department of Energy by Battelle [DE-AC05-76RL01830]; Department of Energy's Office of Biological and Environmental Research FX This work was partially supported by the startup fund from the University of Texas-Pan American as well as the National Science Foundation under DMR grant #0934157 (PREM-UTPA/UMN-Science and Engineering of Polymeric and Nanoparticle-based Materials for Electronic and Structural Applications). The Pacific Northwest National Laboratory (PNNL) is operated for the U.S. Department of Energy by Battelle under Contract DE-AC05-76RL01830. A portion of the research was performed on an instrument (PPMS) housed within the Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. NR 47 TC 12 Z9 12 U1 5 U2 86 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2040-3364 EI 2040-3372 J9 NANOSCALE JI Nanoscale PY 2013 VL 5 IS 11 BP 4720 EP 4728 DI 10.1039/c3nr00825h PG 9 WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 145IL UT WOS:000319008700020 PM 23595132 ER PT J AU Lu, J Qin, Y Du, P Luo, XY Wu, TP Ren, Y Wen, JG Miller, DJ Miller, JT Amine, K AF Lu, Jun Qin, Yan Du, Peng Luo, Xiangyi Wu, Tianpin Ren, Yang Wen, Jianguo Miller, Dean J. Miller, Jeffrey T. Amine, Khalil TI Synthesis and characterization of uniformly dispersed Fe3O4/Fe nanocomposite on porous carbon: application for rechargeable Li-O-2 batteries SO RSC ADVANCES LA English DT Article ID LI-AIR BATTERIES; LITHIUM-OXYGEN BATTERY; LI/AIR BATTERIES; CATHODE CATALYSTS; HIGH-CAPACITY; HIGH-POWER; ELECTRODE; REDUCTION; DISCHARGE; ELECTROCHEMISTRY AB Uniformly dispersed core-shelled Fe/Fe3O4 nanocomposite on porous carbon was synthesized via a wet-chemistry approach, which was tested as a cathode material in rechargeable Li-O-2 battery, showing highly active catalytic effect towards the electrochemical reactions, of particular, oxygen reduction reaction. XPS data showed the oxygen reduction reaction took place on the surface of the catalyst during discharge of the cell. Both XRD and XPS data demonstrated that lithium peroxide partook in the reversible reactions in the Li-O-2 cell with a TEGDME-based electrolyte. C1 [Lu, Jun; Qin, Yan; Du, Peng; Luo, Xiangyi; Miller, Jeffrey T.; Amine, Khalil] Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA. [Wu, Tianpin; Ren, Yang] Argonne Natl Lab, Xray Sci Div, Adv Photon Source, Lemont, IL 60439 USA. [Wen, Jianguo; Miller, Dean J.] Argonne Natl Lab, Electron Microscopy Ctr, Div Mat Sci, Lemont, IL 60439 USA. [Luo, Xiangyi] Univ Utah, Dept Met Engn, Salt Lake City, UT 84112 USA. RP Lu, J (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Lemont, IL 60439 USA. EM amine@anl.gov RI Du, Peng/F-8336-2013; Amine, Khalil/K-9344-2013; Luo, Xiangyi/N-4709-2014; Luo, Xiangyi/K-6058-2015 OI Luo, Xiangyi/0000-0002-4817-1461; Luo, Xiangyi/0000-0002-4817-1461 FU U.S. Department of Energy; FreedomCAR; Vehicle Technologies Office; Department of Energy (DOE) Office of Energy Efficiency and Renewable Energy (EERE) Postdoctoral Research Award under the EERE Vehicles Technology Program; Oak Ridge Associated Universities (ORAU) under DOE [DE-AC05-06OR23100]; DOE Office of Science-Basic Energy Sciences [DE-AC02-06CH11357] FX Research at Argonne National Laboratory was funded by the U.S. Department of Energy, FreedomCAR and Vehicle Technologies Office. J. Lu was supported by the Department of Energy (DOE) Office of Energy Efficiency and Renewable Energy (EERE) Postdoctoral Research Award under the EERE Vehicles Technology Program administered by the Oak Ridge Institute for Science and Education (ORISE) for the DOE. ORISE is managed by Oak Ridge Associated Universities (ORAU) under DOE contract number DE-AC05-06OR23100. The SEM and TEM analysis was performed at the Electron Microscopy Center (EMC), which is supported by the DOE Office of Science-Basic Energy Sciences under contract DE-AC02-06CH11357. Use of the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under contract No. DE-AC02-06CH11357. MRCAT operations are supported by the Department of Energy and the MRCAT member institutions. NR 48 TC 40 Z9 40 U1 12 U2 114 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2046-2069 J9 RSC ADV JI RSC Adv. PY 2013 VL 3 IS 22 BP 8276 EP 8285 DI 10.1039/c3ra40451j PG 10 WC Chemistry, Multidisciplinary SC Chemistry GA 144LM UT WOS:000318940800025 ER PT J AU Ryu, WH Kim, DH Kang, SH Kwon, HS AF Ryu, Won-Hee Kim, Dong-Han Kang, Sun-Ho Kwon, Hyuk-Sang TI Electrochemical properties of nanosized Li-rich layered oxide as positive electrode materials for Li-Ion batteries SO RSC ADVANCES LA English DT Article ID LITHIUM BATTERIES; CATHODE MATERIALS; CELLS; GITT; PERFORMANCE; LICOO2; EIS; MN; NI AB A nanosized Li-rich layered oxide/carbon composite material is successfully prepared by simple ball milling pulverization of microsphere-shaped Li-rich layered oxide materials with conductive carbon. The nanosized Li-rich layered oxide/carbon composite electrode exhibits a high 1st discharge capacity of 250 mAh g(-1) with an excellent rate capability at high current density. The composite also reduces the internal resistance from oxygen release during the electrochemical activation of Li2MnO3. The improvement in the electrochemical performance of nanosized Li-rich layered oxide/carbon composite materials primarily occurs because the nanosized particles facilitate the diffusion of Li within the structure and provide innumerable reaction sites with lithium. Furthermore, the electronic conductivity of the active material is effectively enhanced by the carbon coating on the particles. In addition, unique effects of ball milling on the electrochemical properties of the Li-rich layered oxides are observed: (i) pre-activation of the Li2MnO3 component and (ii) gradual electrochemical activation under 4.3 V during cycling. Adverse effects on the electrochemical stability of the nanosized Li-rich layered oxide are also discussed, and these adverse effects mainly arise due to (i) the structural deformation of hexagonal ordering, (ii) the growth of the spinel component and (iii) the insufficient formation of a protective NiF2 layer on the surface of the active material. C1 [Ryu, Won-Hee; Kwon, Hyuk-Sang] Korea Adv Inst Sci & Technol, Dept Mat Sci & Engn, Taejon 305701, South Korea. [Ryu, Won-Hee; Kim, Dong-Han; Kang, Sun-Ho] Argonne Natl Lab, Div Chem Engn, Argonne, IL 60439 USA. RP Ryu, WH (reprint author), Korea Adv Inst Sci & Technol, Dept Mat Sci & Engn, Taejon 305701, South Korea. EM sh0816.kang@samsung.com; hskwon@kaist.ac.kr RI Kwon, Hyuk Sang/C-1889-2011; Ryu, Won-Hee/F-8375-2014 OI Ryu, Won-Hee/0000-0002-0203-2992 FU Basic Science Research Program through the National Research Foundation of Korea (NRF); Ministry of Education, Science and Technology [NRF-2010-0024752]; Center for Inorganic Photovoltaic Materials [2012-0001167]; Korea government (MEST); BK21 Program of the Korea Ministry of Knowledge Economy FX This research was supported by the Basic Science Research Program through the National Research Foundation of Korea (NRF), which is funded by the Ministry of Education, Science and Technology (NRF-2010-0024752). The work was partially supported by the Center for Inorganic Photovoltaic Materials (2012-0001167) grant funded by the Korea government (MEST) and also by the BK21 Program of the Korea Ministry of Knowledge Economy. NR 33 TC 14 Z9 14 U1 4 U2 84 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2046-2069 J9 RSC ADV JI RSC Adv. PY 2013 VL 3 IS 22 BP 8527 EP 8534 DI 10.1039/c3ra40377g PG 8 WC Chemistry, Multidisciplinary SC Chemistry GA 144LM UT WOS:000318940800056 ER PT J AU Sakai, VG Khodadadi, S Cicerone, MT Curtis, JE Sokolov, AP Roh, JH AF Sakai, Victoria Garcia Khodadadi, Sheila Cicerone, Marcus T. Curtis, Joseph E. Sokolov, Alexei P. Roh, Joon Ho TI Solvent effects on protein fast dynamics: implications for biopreservation SO SOFT MATTER LA English DT Article ID NEUTRON-SCATTERING; MOLECULAR-DYNAMICS; HYDRATION WATER; MICROSCOPIC INSIGHTS; TREHALOSE; GLYCEROL; LYSOZYME; TRANSITION; MYOGLOBIN; GLASS AB In the context of biopreservation, we study the influence of water, glycerol and trehalose on the ps-ns dynamics of lyzosyme using neutron scattering. Results indicate that the choice of bioprotectant depends on the storage temperature; glycerol is the most effective for low temperatures and trehalose for high temperatures. C1 [Sakai, Victoria Garcia] Rutherford Appleton Lab, ISIS Neutron & Muon Facil, Sci & Technol Facil Council, Didcot OX11 0QX, Oxon, England. [Khodadadi, Sheila; Curtis, Joseph E.] NIST, NIST Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Cicerone, Marcus T.] NIST, Polymers Div, Gaithersburg, MD 20899 USA. [Sokolov, Alexei P.] Oak Ridge Natl Lab, Chem Sci Div, Oak Ridge, TN 37831 USA. [Sokolov, Alexei P.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Roh, Joon Ho] Univ Akron, Akron, OH 44325 USA. RP Sakai, VG (reprint author), Rutherford Appleton Lab, ISIS Neutron & Muon Facil, Sci & Technol Facil Council, Didcot OX11 0QX, Oxon, England. EM Victoria.garcia-sakai@stfc.ac.uk; cicerone@nist.gov; joseph.curtis@nist.gov; sokolov@utk.edu; joonho.roh.ctr.ks@nrl.navy.mil OI Garcia Sakai, Victoria/0000-0001-6570-4218 NR 33 TC 13 Z9 13 U1 4 U2 48 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1744-683X J9 SOFT MATTER JI Soft Matter PY 2013 VL 9 IS 22 BP 5336 EP 5340 DI 10.1039/c3sm50492a PG 5 WC Chemistry, Physical; Materials Science, Multidisciplinary; Physics, Multidisciplinary; Polymer Science SC Chemistry; Materials Science; Physics; Polymer Science GA 144MZ UT WOS:000318945100003 ER PT J AU Hur, SM Frischknecht, AL Huber, DL Fredrickson, GH AF Hur, Su-Mi Frischknecht, Amalie L. Huber, Dale L. Fredrickson, Glenn H. TI Self-assembly in a mixed polymer brush with inhomogeneous grafting density composition SO SOFT MATTER LA English DT Article ID CONSISTENT-FIELD THEORY; MICROPHASE SEPARATION; BLOCK-COPOLYMER; SIMULATIONS; MORPHOLOGY; GRADIENTS; MEMORY AB While theoretical and numerical studies have shown the possibility of obtaining long-range ordering from the self-assembly of A-B binary mixed brushes similar to diblock copolymer thin films, such ordered patterns are not currently obtainable experimentally. In addition, most experimental observations of mixed brushes show relatively short range order with many defective structures. One explanation for poor microdomain ordering in experimental mixed brushes is a strong correlation between the spatial distribution of the grafting points and the self-assembly. To investigate this relationship in detail, we use self-consistent field theory (SCFT) simulations to study the phase-separated morphologies of melt mixed brushes with spatially varying grafting density compositions. Variations in the grafting density composition are implemented by modulating the grafting chain end distribution function to locally control the ratio of A and B chains attached to the surface, while maintaining uniform total grafting density. Three different types of grafting density composition variations are investigated: a linear ramping of the grafting density composition, deterministic sinusoidal variations, and random fluctuations with various correlation lengths and strengths. The resulting patterns in the micro-phase separated brush are seen to depend sensitively on both the wavelengths and amplitudes of the imposed grafting density fluctuations. C1 [Hur, Su-Mi; Fredrickson, Glenn H.] Univ Calif Santa Barbara, Dept Chem Engn, Santa Barbara, CA 93106 USA. [Frischknecht, Amalie L.; Huber, Dale L.] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA. [Fredrickson, Glenn H.] Univ Calif Santa Barbara, Dept Mat, Santa Barbara, CA 93106 USA. [Fredrickson, Glenn H.] Univ Calif Santa Barbara, Mat Sci Lab, Santa Barbara, CA 93106 USA. RP Fredrickson, GH (reprint author), Univ Calif Santa Barbara, Dept Chem Engn, Santa Barbara, CA 93106 USA. EM ghf@mrl.ucsb.edu RI Frischknecht, Amalie/N-1020-2014; Huber, Dale/A-6006-2008 OI Frischknecht, Amalie/0000-0003-2112-2587; Huber, Dale/0000-0001-6872-8469 FU U.S. Department of Energy [DE-AC04-94AL85000]; Sandia LDRD program; MARCO Center on Functional Engineered Nano Architectonics (FENA) FX This work was performed, in part, at the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences user facility. Sandia National Laboratories is a multi-program laboratory operated by Sandia Corporation, a Lockheed-Martin Company, for the U.S. Department of Energy under Contract no. DE-AC04-94AL85000. Partial support was also provided from the Sandia LDRD program and from the MARCO Center on Functional Engineered Nano Architectonics (FENA) and computer resources were provided by the Center for Scientific Computing at UCSB, a partnership between CNSI and MRL: an NSF MRSEC (DMR-1121053). NR 29 TC 7 Z9 7 U1 3 U2 55 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1744-683X J9 SOFT MATTER JI Soft Matter PY 2013 VL 9 IS 22 BP 5341 EP 5354 DI 10.1039/c3sm50173f PG 14 WC Chemistry, Physical; Materials Science, Multidisciplinary; Physics, Multidisciplinary; Polymer Science SC Chemistry; Materials Science; Physics; Polymer Science GA 144MZ UT WOS:000318945100004 ER PT J AU Meng, D Kumar, SK Cheng, SF Grest, GS AF Meng, Dong Kumar, Sanat K. Cheng, Shengfeng Grest, Gary S. TI Simulating the miscibility of nanoparticles and polymer melts SO SOFT MATTER LA English DT Article ID MOLECULAR-DYNAMICS SIMULATION; MODEL ATHERMAL MIXTURES; SELF-EXCLUDING POLYMERS; PHASE-BEHAVIOR; COMPUTER-SIMULATIONS; NANOCOMPOSITES; MATRIX; PARTICLES; COLLOIDS; SYSTEMS AB While the miscibility and spatial dispersion of nanoparticles (NPs) in a polymer melt critically affects the properties of the resulting nanocomposite, little simulation work exists on understanding this critical issue. We use isothermal-isobaric ensemble simulations and show that larger NPs disperse more easily than small NPs, implying the relative dominance of NP-polymer attractions over depletion-induced inter-NP attractions. Similarly, polymer chain length only plays a secondary role, probably because the entropic, depletion-induced inter-NP attractions only occur over length scales comparable to the correlation length in the melt, namely the segment size, sigma. Importantly, no NP self-assembly is observed, and the only transition that occurs for polymer systems with large enough NPs (sigma(NP) >= 6 sigma) is of a purely, first-order solid-fluid type. This result follows from the fact that the range of effective attractions between the NPs, delta = sigma/sigma(NP), is short enough to preclude a vapor-liquid transition. This finding is given more weight since an equivalent sticky sphere model can reproduce the essence of our simulations. The observed behavior is captured by an effective two-body, polymer-mediated, inter-NP interaction potential, a surprising result in light of conventional wisdom in this field which implies the importance of many body effects. C1 [Meng, Dong; Kumar, Sanat K.] Columbia Univ, Dept Chem Engn, New York, NY 10027 USA. [Cheng, Shengfeng; Grest, Gary S.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Kumar, SK (reprint author), Columbia Univ, Dept Chem Engn, New York, NY 10027 USA. EM sk2794@columbia.edu RI Meng, Dong/D-8328-2014; OI Meng, Dong/0000-0003-1763-6411; Cheng, Shengfeng/0000-0002-6066-2968 FU National Science Foundation [CBET-1033168]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; Advanced Scientific Computing Research (ASCR) Leadership Computing Challenge (ALCC); Laboratory Directed Research and Development (LDRD); National Institute for Nano-Engineering at Sandia National Laboratories; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Financial support from the National Science Foundation (CBET-1033168) is gratefully acknowledged. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract no. DE-AC02-05CH11231 and the Advanced Scientific Computing Research (ASCR) Leadership Computing Challenge (ALCC). This work was supported in part by the Laboratory Directed Research and Development (LDRD) and the National Institute for Nano-Engineering at Sandia National Laboratories. This work was performed, in part, at the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences user facility. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 67 TC 16 Z9 16 U1 7 U2 64 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1744-683X J9 SOFT MATTER JI Soft Matter PY 2013 VL 9 IS 22 BP 5417 EP 5427 DI 10.1039/c3sm50460c PG 11 WC Chemistry, Physical; Materials Science, Multidisciplinary; Physics, Multidisciplinary; Polymer Science SC Chemistry; Materials Science; Physics; Polymer Science GA 144MZ UT WOS:000318945100012 ER PT S AU Reichhardt, C Nussinov, Z Reichhardt, CJO AF Reichhardt, C. Nussinov, Z. Reichhardt, C. J. Olson BE Chauhan, AK Murli, C Gadkari, SC TI Connecting Jamming and Depinning Transitions SO SOLID STATE PHYSICS, VOL 57 SE AIP Conference Proceedings LA English DT Proceedings Paper CT 57th DAE Solid State Physics Symposium CY DEC 03-07, 2012 CL Indian Inst Technol, Bombay, INDIA SP Gov India, Dept Atom Energy (DAE), Board Res Nucl Sci (BRNS) HO Indian Inst Technol DE jamming; pinning; peak effect; granular matter ID FLUX-LINE-LATTICE; DYNAMICS AB We examine a system of binary disks that is known to exhibit a jamming transition at a well defined density termed point J. We add quenched disorder and measure the external force needed to depin the disks or send them into motion as a function of disk density. We find a rich variety of depinning behaviors. For small amounts of disorder, only the jammed or stiff phases are pinned. For strong disorder, disks in unjammed samples with densities well below jamming are more strongly pinned than disks in samples at densities close to the jamming transition. We also discuss connections to the peak effect for depinning in vortex systems. C1 [Reichhardt, C.; Reichhardt, C. J. Olson] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Reichhardt, C (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM reichhardt@lanl.gov NR 12 TC 0 Z9 0 U1 1 U2 7 PU AMER INST PHYSICS PI MELVILLE PA 2 HUNTINGTON QUADRANGLE, STE 1NO1, MELVILLE, NY 11747-4501 USA SN 0094-243X BN 978-0-7354-1133-3 J9 AIP CONF PROC PY 2013 VL 1512 BP 7 EP 10 DI 10.1063/1.4790891 PG 4 WC Physics, Applied; Physics, Condensed Matter SC Physics GA BEL78 UT WOS:000317266700001 ER PT B AU McMahon, JM Gray, SK Schatz, GC AF McMahon, Jeffrey M. Gray, Stephen K. Schatz, George C. BE Taflove, A Oskooi, A Johnson, SG TI FDTD Computation of the Non local Optical Properties of Arbitrarily Shaped Nanostructures SO ADVANCES IN FDTD COMPUTATIONAL ELECTRODYNAMICS: PHOTONICS AND NANOTECHNOLOGY SE Artech House Antennas and Propagation Series LA English DT Article; Book Chapter ID LONGITUDINAL PLASMONS; SINGLE-MOLECULE; METALLIC-FILMS; NANOPARTICLES; MEDIA; SCATTERING; RESONANCE; SPHERES C1 [McMahon, Jeffrey M.] Univ Illinois, Inst Condensed Matter Theory, Urbana, IL 61801 USA. [Gray, Stephen K.] Argonne Natl Lab, Argonne, IL 60439 USA. [Gray, Stephen K.] Argonne Natl Lab, Ctr Nanoscale Mat, Theory & Modeling Grp, Argonne, IL 60439 USA. [Gray, Stephen K.] Amer Phys Soc, College Pk, MD USA. [Schatz, George C.] Northwestern Univ, Evanston, IL USA. [Schatz, George C.] MIT, Cambridge, MA 02139 USA. RP McMahon, JM (reprint author), Univ Illinois, Inst Condensed Matter Theory, Urbana, IL 61801 USA. RI Wessels, Bruce/B-7541-2009; Taflove, Allen/B-7275-2009 NR 43 TC 0 Z9 0 U1 0 U2 1 PU ARTECH HOUSE PI NORWOOD PA 685 CANTON ST, NORWOOD, MA 02062 USA BN 978-1-60807-170-8 J9 ARTECH HSE ANTENN PR PY 2013 BP 185 EP 207 PG 23 WC Mathematics, Interdisciplinary Applications; Optics; Telecommunications SC Mathematics; Optics; Telecommunications GA BET91 UT WOS:000318121700010 ER PT B AU Chen, HN McMahon, JM Ratner, MA Schatz, GC AF Chen, Hanning McMahon, Jeffrey M. Ratner, Mark A. Schatz, George C. BE Taflove, A Oskooi, A Johnson, SG TI Classical Electrodynamics Coupled to Quantum Mechanics for Calculation of Molecular Optical Properties: An RT-TDDFT/FDTD Approach SO ADVANCES IN FDTD COMPUTATIONAL ELECTRODYNAMICS: PHOTONICS AND NANOTECHNOLOGY SE Artech House Antennas and Propagation Series LA English DT Article; Book Chapter ID PHOTOINDUCED ELECTRON-TRANSFER; ENHANCED RAMAN-SPECTROSCOPY; DENSITY-FUNCTIONAL THEORY; SENSITIZED SOLAR-CELLS; METAL NANOPARTICLES; RESPONSE PROPERTIES; GOLD NANOPARTICLES; TIO2 FILM; SILVER; APPROXIMATION C1 [Chen, Hanning] George Washington Univ, Washington, DC 20052 USA. [Chen, Hanning] Northwestern Univ, Argonne Natl Lab, Solar Energy Res Ctr, Evanston, IL 60208 USA. [McMahon, Jeffrey M.] Univ Illinois, Inst Condensed Matter Theory, Urbana, IL 61801 USA. [Ratner, Mark A.; Schatz, George C.] Northwestern Univ, Evanston, IL USA. [Ratner, Mark A.] Northwestern ISEN, Initiat Sustainabil & Energy, Evanston, IL USA. [Ratner, Mark A.] Aarhus Univ, DK-8000 Aarhus C, Denmark. [Ratner, Mark A.] Univ Munich, Munich, Germany. [Ratner, Mark A.] NYU, New York, NY 10003 USA. [Schatz, George C.] MIT, Cambridge, MA 02139 USA. RP Chen, HN (reprint author), George Washington Univ, Washington, DC 20052 USA. RI Wessels, Bruce/B-7541-2009; Taflove, Allen/B-7275-2009 NR 53 TC 0 Z9 0 U1 0 U2 11 PU ARTECH HOUSE PI NORWOOD PA 685 CANTON ST, NORWOOD, MA 02062 USA BN 978-1-60807-170-8 J9 ARTECH HSE ANTENN PR PY 2013 BP 209 EP 231 PG 23 WC Mathematics, Interdisciplinary Applications; Optics; Telecommunications SC Mathematics; Optics; Telecommunications GA BET91 UT WOS:000318121700011 ER PT J AU Fongkaew, I T-Thienprasert, J Singh, DJ Du, MH Limpijumnong, S AF Fongkaew, Ittipon T-Thienprasert, Jiraroj Singh, D. J. Du, M. -H. Limpijumnong, Sukit TI First principles calculations of Hydrogen-Titanium vacancy complexes in SrTiO3 SO CERAMICS INTERNATIONAL LA English DT Article; Proceedings Paper CT 8th Asian Meeting on Electroceramics (AMEC) CY JUL 01-05, 2012 CL MALAYSIA SP Off Naval Res Global DE SrTiO3; Hydrogen; Vacancy; First principles calculations ID STRONTIUM-TITANATE; ULTRASOFT PSEUDOPOTENTIALS; STRETCHING VIBRATIONS; O-H; SPECTROSCOPY; IMPURITIES; FILMS AB Hydrogen has been reported to serve exclusively as a donor in many oxides, including SrTiO3. In a perfect crystal, a proton stays near an O atom, forming a strong O-H bond. In the presence of cation vacancies, i.e., Sr vacancy and Ti vacancy, protons prefer to electrically passivate the cation vacancies by forming strong bonds with the O atoms surrounding the vacancy. These result in the formation of nH-V-Sr and nH-V-Ti complexes. Based on first principles density functional calculations, local configurations and vibration signatures of nH-V-Sr complexes and their vibrational signatures have been previously reported [T-Thienprasert et al., Identification of hydrogen defects in SrTiO3 by first-principles local vibration mode calculations, Physical Review B 85, 125205 (2012)]. Here, we report the computational results for nH-V-Ti complexes and compare the results with infrared measurements reported in the literatures. (C) 2012 Elsevier Ltd and Techna Group S.r.l. All rights reserved. C1 [Fongkaew, Ittipon; Limpijumnong, Sukit] Suranaree Univ Technol, Sch Phys, Nakhon Ratchasima 30000, Thailand. [Fongkaew, Ittipon; T-Thienprasert, Jiraroj; Limpijumnong, Sukit] Thailand Ctr Excellence Phys ThEP Ctr, Commiss Higher Educ, Bangkok 10400, Thailand. [T-Thienprasert, Jiraroj] Kasetsart Univ, Fac Sci, Dept Phys, Bangkok 10900, Thailand. [Singh, D. J.; Du, M. -H.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Limpijumnong, S (reprint author), Suranaree Univ Technol, Sch Phys, Nakhon Ratchasima 30000, Thailand. EM sukit@sut.ac.th RI Du, Mao-Hua/B-2108-2010 OI Du, Mao-Hua/0000-0001-8796-167X NR 29 TC 2 Z9 2 U1 1 U2 26 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0272-8842 EI 1873-3956 J9 CERAM INT JI Ceram. Int. PY 2013 VL 39 SU 1 BP S273 EP S276 DI 10.1016/j.ceramint.2012.10.076 PG 4 WC Materials Science, Ceramics SC Materials Science GA 141SU UT WOS:000318747600053 ER PT J AU Tanabe, KK Siladke, NA Broderick, EM Kobayashi, T Goldston, JF Weston, MH Farha, OK Hupp, JT Pruski, M Mader, EA Johnson, MJA Nguyen, ST AF Tanabe, Kristine K. Siladke, Nathan A. Broderick, Erin M. Kobayashi, Takeshi Goldston, Jennifer F. Weston, Mitchell H. Farha, Omar K. Hupp, Joseph T. Pruski, Marek Mader, Elizabeth A. Johnson, Marc J. A. Nguyen, SonBinh T. TI Stabilizing unstable species through single-site isolation: a catalytically active Ta-V trialkyl in a porous organic polymer SO CHEMICAL SCIENCE LA English DT Article ID HIGH-SURFACE-AREA; AROMATIC FRAMEWORK; HYDROGEN STORAGE; INORGANIC OXIDES; COMPLEXES; TANTALUM; CATALYSIS; NETWORKS; GAS; METATHESIS AB A catechol-functionalized porous organic polymer (POP) has been successfully metallated with a Ta-V trialkyl and remains thermally and structurally robust. The resulting POP-supported (catecholato)Ta-V trialkyl sites remain accessible to small molecules and can undergo reactions to yield stable, monomeric complexes that are quite different from those observed with the homogeneous analogues. Using a combination of reactivity studies, high-resolution solid-state NMR spectroscopy, and X-ray absorption spectroscopy (XAS), we are able to precisely determine the functionality and coordination environment of the active (catecholato)Ta-V trialkyl site and its products in reactions with Bronsted acids. Additionally, the Ta-metallated POP was found to have enhanced catalytic activity in the hydrogenation of cyclohexene and toluene relative to a homogeneous analogue. C1 [Tanabe, Kristine K.; Siladke, Nathan A.; Broderick, Erin M.; Hupp, Joseph T.; Mader, Elizabeth A.; Johnson, Marc J. A.; Nguyen, SonBinh T.] Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA. [Kobayashi, Takeshi; Goldston, Jennifer F.; Pruski, Marek] US DOE, Ames Lab, Ames, IA 50011 USA. [Goldston, Jennifer F.; Pruski, Marek] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. [Weston, Mitchell H.; Farha, Omar K.; Hupp, Joseph T.; Nguyen, SonBinh T.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Weston, Mitchell H.; Farha, Omar K.; Hupp, Joseph T.; Nguyen, SonBinh T.] Northwestern Univ, Int Inst Nanotechnol, Evanston, IL 60208 USA. RP Mader, EA (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Lemont, IL 60439 USA. EM mader@anl.gov; mjjohnson@anl.gov; stn@anl.gov RI Nguyen, SonBinh/C-1682-2014 OI Nguyen, SonBinh/0000-0002-6977-3445 FU U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-06CH11357]; U.S. DOE [DE-AC02-06CH11357]; U.S. DOE, Office of Basic Energy Sciences [AL-03-380-011, W-7405-Eng-82]; DTRA [HDTRA1-10-1-0023] FX We thank S. C. Browne, N. David, and L. M. Fenton for synthesizing some of the starting materials used in this work. We thank Dr. M. S. Ferrandon for help with the initial catalysis setup and Dr. S. J. Lopykinski for help with the gas chromatography setup. We thank Drs. J. T. Miller and A. S. Hock for helpful discussions. Work carried out at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under contract DE-AC02-06CH11357. Use of the Advanced Photon Source, a User Facility operated for the U.S. Department of Energy (DOE), Office of Science by Argonne National Laboratory, was also supported by the U.S. DOE under Contract no. DE-AC02-06CH11357. Ames Laboratory's work was supported through the U.S. DOE, Office of Basic Energy Sciences, through Catalysis Science Grant AL-03-380-011 and under Contract W-7405-Eng-82. S. T. N., J. T. H., and O. K. F. additionally acknowledge DTRA (Agreement HDTRA1-10-1-0023) for support. NR 58 TC 23 Z9 23 U1 7 U2 59 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2041-6520 J9 CHEM SCI JI Chem. Sci. PY 2013 VL 4 IS 6 BP 2483 EP 2489 DI 10.1039/c3sc22268c PG 7 WC Chemistry, Multidisciplinary SC Chemistry GA 139CS UT WOS:000318559700024 ER PT J AU Flannery, DJ Modzeleski, W Kretschmar, JM AF Flannery, Daniel J. Modzeleski, William Kretschmar, Jeff M. TI Violence and School Shootings SO CURRENT PSYCHIATRY REPORTS LA English DT Article DE School violence; Shootings; Firearms; Homicide; Threat assessment; Mental health; Rampage; Profiling; Targeted; Prevention; Treatment; Survivors; Trauma; Child and adolescent disorders; Psychiatry ID PSYCHOLOGICAL TRAUMA; THREAT ASSESSMENT; UNITED-STATES; SUICIDE; ADOLESCENTS; BEHAVIORS; EXPOSURE; CONTRIBUTORS; SAMPLE; RISK AB Multiple-homicide school shootings are rare events, but when they happen they significantly impact individuals, the school and the community. We focus on multiple-homicide incidents and identified mental health issues of shooters. To date, studies of school shootings have concluded that no reliable profile of a shooter exists, so risk should be assessed using comprehensive threat assessment protocols. Existing studies primarily utilize retrospective case histories or media accounts. The field requires more empirical and systematic research on all types of school shootings including single victim incidents, those that result in injury but not death and those that are successfully averted. We discuss current policies and practices related to school shootings and the role of mental health professionals in assessing risk and supporting surviving victims. C1 [Flannery, Daniel J.; Kretschmar, Jeff M.] Case Western Reserve Univ, Mandel Sch Appl Social Sci, Cleveland, OH 44106 USA. [Modzeleski, William] US DOE, Off Safe & Drug Free Sch, Washington, DC 20585 USA. RP Flannery, DJ (reprint author), Case Western Reserve Univ, Mandel Sch Appl Social Sci, 11402 Bellflower Rd, Cleveland, OH 44106 USA. EM daniel.flannery@case.edu; WModzeleski@gmail.com; jeff.kretschmar@case.edu NR 44 TC 7 Z9 7 U1 10 U2 71 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1523-3812 J9 CURR PSYCHIAT REP JI Curr. Psychiatry Rep. PD JAN PY 2013 VL 15 IS 1 AR 6 DI 10.1007/s11920-012-0331-6 PG 7 WC Psychiatry SC Psychiatry GA 141XM UT WOS:000318759800001 PM 23254623 ER PT J AU Aaron, D Sun, CN Bright, M Papandrew, AB Mench, MM Zawodzinski, TA AF Aaron, Douglas Sun, Che-Nan Bright, Michael Papandrew, Alexander B. Mench, Matthew M. Zawodzinski, Thomas A. TI In Situ Kinetics Studies in All-Vanadium Redox Flow Batteries SO ECS ELECTROCHEMISTRY LETTERS LA English DT Article ID PEM FUEL-CELLS; REFERENCE ELECTRODE AB We report results of polarization measurements resolved for the negative and positive electrodes of vanadium redox batteries (VRBs) using a dynamic hydrogen electrode in an operating battery cell. Electrochemical experiments with symmetric electrolyte feeds were also performed. Greater kinetic polarization is observed at the negative (V3/2+) electrode compared to the positive electrode (V5/4+), in contrast with previously reported ex situ measurements. For the positive electrode, the polarization in the low-current regime was modest and was not kinetically controlled. The relative rates of reaction are a surprise since it might be expected that the V3/2+ redox reaction is a simple outer-sphere electron transfer. (c) 2013 The Electrochemical Society. All rights reserved. C1 [Aaron, Douglas; Bright, Michael; Papandrew, Alexander B.; Zawodzinski, Thomas A.] Univ Tennessee, Knoxville, TN 37996 USA. [Sun, Che-Nan; Zawodzinski, Thomas A.] Oak Ridge Natl Lab, Phys Chem Mat Grp, Oak Ridge, TN 37831 USA. [Mench, Matthew M.] Univ Tennessee, Dept Mech Aerosp & Biomed Engn, Knoxville, TN 37996 USA. [Mench, Matthew M.] Oak Ridge Natl Lab, Emiss & Catalysis Res Grp, Oak Ridge, TN 37831 USA. RP Aaron, D (reprint author), Univ Tennessee, Knoxville, TN 37996 USA. EM tzawodzi@utk.edu RI Sun, Che-Nan/I-3871-2013 NR 13 TC 38 Z9 38 U1 6 U2 101 PU ELECTROCHEMICAL SOC INC PI PENNINGTON PA 65 SOUTH MAIN STREET, PENNINGTON, NJ 08534 USA SN 2162-8726 J9 ECS ELECTROCHEM LETT JI ECS Electrochem. Lett. PY 2013 VL 2 IS 3 BP A29 EP A31 DI 10.1149/2.001303eel PG 3 WC Electrochemistry; Materials Science, Multidisciplinary SC Electrochemistry; Materials Science GA 139AQ UT WOS:000318554100001 ER PT J AU Sun, CN Delnick, FM Aaron, DS Papandrew, AB Mench, MM Zawodzinski, TA AF Sun, Che-Nan Delnick, F. M. Aaron, D. S. Papandrew, A. B. Mench, M. M. Zawodzinski, T. A. TI Probing Electrode Losses in All-Vanadium Redox Flow Batteries with Impedance Spectroscopy SO ECS ELECTROCHEMISTRY LETTERS LA English DT Article ID CELL AB We report on single-electrode electrochemical impedance spectroscopy studies of an all-vanadium redox battery using a dynamic hydrogen reference electrode. The negative electrode, comprising the V2+/V3+ couple, contributes approximately 80% of the total cell overpotential during discharge. The impedance spectra measured at the negative electrode exhibit high-frequency, semicircular arcs which correspond to the double layer capacitance in parallel with a faradaic resistance. The faradaic resistance decreases in magnitude with increasing polarization. Integration of the current-dependent faradaic resistance quantifies the fraction of the overvoltage that is attributed to the kinetic limitations of the charge transfer reaction. (c) 2013 The Electrochemical Society. All rights reserved. C1 [Sun, Che-Nan; Mench, M. M.; Zawodzinski, T. A.] Oak Ridge Natl Lab, Emiss & Catalysis Res Grp, Phys Chem Mat Grp, Oak Ridge, TN 37831 USA. [Delnick, F. M.] Sandia Natl Labs, Power Sources Technol Grp, Albuquerque, NM 87185 USA. [Aaron, D. S.; Papandrew, A. B.; Mench, M. M.; Zawodzinski, T. A.] Univ Tennessee, Dept Mech Aerosp & Biomed Engn, Dept Chem & Biomol Engn, Knoxville, TN 37996 USA. RP Sun, CN (reprint author), Oak Ridge Natl Lab, Emiss & Catalysis Res Grp, Phys Chem Mat Grp, Oak Ridge, TN 37831 USA. EM sunc@ornl.gov RI Sun, Che-Nan/I-3871-2013 FU US Department of Energy Office of Electricity Storage Systems Program; University of Tennessee Governor's Chair Fund FX The authors gratefully acknowledge the support of the US Department of Energy Office of Electricity Storage Systems Program and the University of Tennessee Governor's Chair Fund for support of this work. NR 15 TC 29 Z9 30 U1 5 U2 67 PU ELECTROCHEMICAL SOC INC PI PENNINGTON PA 65 SOUTH MAIN STREET, PENNINGTON, NJ 08534 USA SN 2162-8726 J9 ECS ELECTROCHEM LETT JI ECS Electrochem. Lett. PY 2013 VL 2 IS 5 BP A43 EP A45 DI 10.1149/2.001305eel PG 3 WC Electrochemistry; Materials Science, Multidisciplinary SC Electrochemistry; Materials Science GA 139BN UT WOS:000318556600001 ER PT J AU Atanasoski, RT Cullen, DA Vernstrom, GD Haugen, GM Atanasoska, LL AF Atanasoski, R. T. Cullen, D. A. Vernstrom, G. D. Haugen, G. M. Atanasoska, L. L. TI A Materials-Based Mitigation Strategy for SU/SD in PEM Fuel Cells: Properties and Performance-Specific Testing of IrRu OER Catalysts SO ECS ELECTROCHEMISTRY LETTERS LA English DT Article ID MEMBRANE AB Catalysts that enable proton exchange membrane fuel cells to weather the damaging conditions experienced during transient periods of fuel starvation have been developed. The addition of minute amounts of iridium and ruthenium to the cathode enhances the oxygen evolution reaction (OER) during start-up/shutdown events, thus lowering the peak cell voltage closer to the onset of water oxidation. The catalyst loadings ranged from 1 to 10 mu g/cm(2), but showed surprisingly high activity and durability. At such low loadings, it is possible to fully integrate the OER catalysts with negligible interference on fuel cell performance and a marginal increase in catalyst cost. (c) 2013 The Electrochemical Society. All rights reserved. C1 [Atanasoski, R. T.; Vernstrom, G. D.; Haugen, G. M.] 3M Co, Fuel Cell Program 3M, St Paul, MN 55144 USA. [Cullen, D. A.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Atanasoska, L. L.] 3M Co, Corp Res Analyt Lab 3M, St Paul, MN 55144 USA. RP Atanasoski, RT (reprint author), 3M Co, Fuel Cell Program 3M, St Paul, MN 55144 USA. EM rtatanasoski@mmm.com RI Cullen, David/A-2918-2015 OI Cullen, David/0000-0002-2593-7866 FU Fuel Cell Technologies Program, Office of Energy Efficiency and Renewable Energy, U.S. Department of Energy [DE-EE0000456]; Oak Ridge National Laboratory's Shared Research Equipment (ShaRE) User Program; Office of Basic Energy Sciences, U.S. Department of Energy FX The MEA assembly and testing by Jimmy Wong and Theresa Watschke is highly appreciated. This work was supported by the Fuel Cell Technologies Program, Office of Energy Efficiency and Renewable Energy, U.S. Department of Energy under Award Number DE-EE0000456.; Research sponsored by Oak Ridge National Laboratory's Shared Research Equipment (ShaRE) User Program, which is sponsored by the Office of Basic Energy Sciences, U.S. Department of Energy. NR 12 TC 5 Z9 5 U1 1 U2 13 PU ELECTROCHEMICAL SOC INC PI PENNINGTON PA 65 SOUTH MAIN STREET, PENNINGTON, NJ 08534 USA SN 2162-8726 J9 ECS ELECTROCHEM LETT JI ECS Electrochem. Lett. PY 2013 VL 2 IS 3 BP F25 EP F28 DI 10.1149/2.006303eel PG 4 WC Electrochemistry; Materials Science, Multidisciplinary SC Electrochemistry; Materials Science GA 139AQ UT WOS:000318554100007 ER PT J AU Aad, G Abajyan, T Abbott, B Abdallah, J Khalek, SA Abdelalim, AA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Acerbi, E Acharya, BS Adamczyk, L Adams, DL Addy, TN Adelman, J Adomeit, S Adragna, P Adye, T Aefsky, S Aguilar-Saavedra, JA Agustoni, M Aharrouche, M Ahlen, SP Ahles, F Ahmad, A Ahsan, M Aielli, G Akdogan, T Akesson, TPA Akimoto, G Akimov, AV Alam, MS Alam, MA Albert, J Albrand, S Aleksa, M Aleksandrov, IN Alessandria, F Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Aliev, M Alimonti, G Alison, J Allbrooke, BMM Allport, PP Allwood-Spiers, SE Almond, J Aloisio, A Alon, R Alonso, A Alonso, F Gonzalez, BA Alviggi, MG Amako, K Amelung, C Ammosov, VV Amorim, A Amram, N Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Anduaga, XS Anger, P Angerami, A Anghinolfi, F Anisenkov, A Anjos, N Annovi, A Antonaki, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Aoun, S Bella, LA Apolle, R Arabidze, G Aracena, I Arai, Y Arce, ATH Arfaoui, S Arguin, JF Arik, E Arik, M Armbruster, AJ Arnaez, O Arnal, V Arnault, C Artamonov, A Artoni, G Arutinov, D Asai, S Asfandiyarov, R Ask, S Asman, B Asquith, L Assamagan, K Astbury, A Aubert, B Auge, E Augsten, K Aurousseau, M Avolio, G Avramidou, R Axen, D Azuelos, G Azuma, Y Baak, MA Baccaglioni, G Bacci, C Bach, AM Bachacou, H Bachas, K Backes, M Backhaus, M Badescu, E Bagnaia, P Bahinipati, S Bai, Y Bailey, DC Bain, T Baines, JT Baker, OK Baker, MD Baker, S Banas, E Banerjee, P Banerjee, S Banfi, D Bangert, A Bansal, V Bansil, HS Barak, L Baranov, SP Galtieri, AB Barber, T Barberio, EL Barberis, D Barbero, M Bardin, DY Barillari, T Barisonzi, M Barklow, T Barlow, N Barnett, BM Barnett, RM Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Barrillon, P Bartoldus, R Barton, AE Bartsch, V Bates, RL Batkova, L Batley, JR Battaglia, A Battistin, M Bauer, F Bawa, HS Beale, S Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, AK Becker, S Beckingham, M Becks, KH Beddall, AJ Beddall, A Bedikian, S Bednyakov, VA Bee, CP Beemster, LJ Begel, M Harpaz, SB Beimforde, M Belanger-Champagne, C Bell, PJ Bell, WH Bella, G Bellagamba, L Bellina, F Bellomo, M Belloni, A Beloborodova, O Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Benoit, M Bensinger, JR Benslama, K Bentvelsen, S Berge, D Kuutmann, EB Berger, N Berghaus, F Berglund, E Beringer, J Bernat, P Bernhard, R Bernius, C Berry, T Bertella, C Bertin, A Bertolucci, F Besana, MI Besjes, GJ Besson, N Bethke, S Bhimji, W Bianchi, RM Bianco, M Biebel, O Bieniek, SP Bierwagen, K Biesiada, J Biglietti, M Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Biscarat, C Bitenc, U Black, KM Blair, 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Buchanan, J Buchholz, P Buckingham, RM Buckley, AG Buda, SI Budagov, IA Budick, B Buescher, V Bugge, L Bulekov, O Bundock, AC Bunse, M Buran, T Burckhart, H Burdin, S Burgess, T Burke, S Busato, E Bussey, P Buszello, CP Butler, B Butler, JM Buttar, CM Butterworth, JM Buttinger, W Byszewski, M Urban, SC Caforio, D Cakir, O Calafiura, P Calderini, G Calfayan, P Calkins, R Caloba, LP Caloi, R Calvet, D Calvet, S Toro, RC Camarri, P Cameron, D Caminada, LM Campana, S Campanelli, M Canale, V Canelli, F Canepa, A Cantero, J Cantrill, R Capasso, L Garrido, MDMC Caprini, I Caprini, M Capriotti, D Capua, M Caputo, R Cardarelli, R Carli, T Carlino, G Carminati, L Caron, B Caron, S Carquin, E Montoya, GDC Carter, AA Carter, JR Carvalho, J Casadei, D Casado, MP Cascella, M Caso, C Hernandez, AMC Castaneda-Miranda, E Gimenez, VC Castro, NF Cataldi, G Catastini, P Catinaccio, A Catmore, JR Cattai, A Cattani, G Caughron, S Cavalleri, P Cavalli, D Cavalli-Sforza, M Cavasinni, V Ceradini, F Cerqueira, AS Cerri, A Cerrito, L Cerutti, F Cetin, SA Chafaq, A Chakraborty, D Chalupkova, I Chan, K Chapleau, B Chapman, JD Chapman, JW Chareyre, E Charlton, DG Chavda, V Barajas, CAC Cheatham, S Chekanov, S Chekulaev, SV Chelkov, GA Chelstowska, MA Chen, C Chen, H Chen, S Chen, X Chen, Y Cheplakov, A El Moursli, RC Chernyatin, V Cheu, E Cheung, SL Chevalier, L Chiefari, G Chikovani, L Childers, JT Chilingarov, A Chiodini, G Chisholm, AS Chislett, RT Chitan, A Chizhov, MV Choudalakis, G Chouridou, S Christidi, IA Christov, A Chromek-Burckhart, D Chu, ML Chudoba, J Ciapetti, G Ciftci, AK Ciftci, R Cinca, D Cindro, V Ciocca, C Ciocio, A Cirilli, M Cirkovic, P Citterio, M Ciubancan, M Clark, A Clark, PJ Clarke, RN Cleland, W Clemens, JC Clement, B Clement, C Coadou, Y Cobal, M Coccaro, A Cochran, J Cogan, JG Coggeshall, J Cogneras, E Colas, J Cole, S Colijn, AP Collins, NJ Collins-Tooth, C Collot, J Colombo, T Colon, G Muino, PC Coniavitis, E Conidi, MC Consonni, SM Consorti, V Constantinescu, S Conta, C Conti, G Conventi, F Cooke, M Cooper, BD Cooper-Sarkar, AM Copic, K Cornelissen, T Corradi, M Corriveau, F Cortes-Gonzalez, A Cortiana, G Costa, G Costa, MJ Costanzo, D Costin, T Cote, D Courneyea, L Cowan, G Cowden, C Cox, BE Cranmer, K Crescioli, F Cristinziani, M Crosetti, G Crepe-Renaudin, S Cuciuc, CM Almenar, CC Donszelmann, TC Curatolo, M Curtis, CJ Cuthbert, C Cwetanski, P Czirr, H Czodrowski, P Czyczula, Z D'Auria, S D'Onofrio, M D'Orazio, A De Sousa, MJDS Da Via, C Dabrowski, W Dafinca, A Dai, T Dallapiccola, C Dam, M Dameri, M Damiani, DS Danielsson, HO Dao, V Darbo, G Darlea, GL Dassoulas, JA Davey, W Davidek, T Davidson, N Davidson, R Davies, E Davies, M Davignon, O Davison, AR Davygora, Y Dawe, E Dawson, I Daya-Ishmukhametova, RK De, K de Asmundis, R De Castro, S De Cecco, S de Graat, J De Groot, N de Jong, P De La Taille, C De la Torre, H De Lorenzi, F de Mora, L De Nooij, L De Pedis, D De Salvo, A De Sanctis, U De Santo, A De Regie, JBD De Zorzi, G Dearnaley, 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Wildt, M. A. Wilhelm, I. Wilkens, H. G. Will, J. Z. Williams, E. Williams, H. H. Willis, W. Willocq, S. Wilson, J. A. Wilson, M. G. Wilson, A. Wingerter-Seez, I. Winkelmann, S. Winklmeier, F. Wittgen, M. Wollstadt, S. J. Wolter, M. W. Wolters, H. Wong, W. C. Wooden, G. Wosiek, B. K. Wotschack, J. Woudstra, M. J. Wozniak, K. W. Wraight, K. Wright, C. Wright, M. Wrona, B. Wu, S. L. Wu, X. Wu, Y. Wulf, E. Wynne, B. M. Xella, S. Xiao, M. Xie, S. Xu, C. Xu, D. Yabsley, B. Yacoob, S. Yamada, M. Yamaguchi, H. Yamamoto, A. Yamamoto, K. Yamamoto, S. Yamamura, T. Yamanaka, T. Yamaoka, J. Yamazaki, T. Yamazaki, Y. Yan, Z. Yang, H. Yang, U. K. Yang, Y. Yang, Z. Yanush, S. Yao, L. Yao, Y. Yasu, Y. Smit, G. V. Ybeles Ye, J. Ye, S. Yilmaz, M. Yoosoofmiya, R. Yorita, K. Yoshida, R. Young, C. Young, C. J. Youssef, S. Yu, D. Yu, J. Yu, J. Yuan, L. Yurkewicz, A. Zabinski, B. Zaidan, R. Zaitsev, A. M. Zajacova, Z. Zanello, L. Zaytsev, A. Zeitnitz, C. Zeman, M. Zemla, A. Zendler, C. Zenin, O. Zenis, T. Zinonos, Z. Zenz, S. Zerwas, D. della Porta, G. Zevi Zhan, Z. Zhang, D. Zhang, H. Zhang, J. Zhang, X. Zhang, Z. Zhao, L. Zhao, T. Zhao, Z. Zhemchugov, A. Zhong, J. Zhou, B. Zhou, N. Zhou, Y. Zhu, C. G. Zhu, H. Zhu, J. Zhu, Y. Zhuang, X. Zhuravlov, V. Zieminska, D. Zimin, N. I. Zimmermann, R. Zimmermann, S. Zimmermann, S. Ziolkowski, M. Zitoun, R. Zivkovic, L. Zmouchko, V. V. Zobernig, G. Zoccoli, A. zur Nedden, M. Zutshi, V. Zwalinski, L. CA ATLAS Collaboration TI Measurements of top quark pair relative differential cross-sections with ATLAS in pp collisions at root s=7 TeV SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID PARTON DISTRIBUTIONS; P(P)OVER-BAR COLLISIONS; T(T)OVER-BAR; SEARCH; JETS AB Measurements are presented of differential cross-sections for top quark pair production in pp collisions at root s = 7 TeV relative to the total inclusive top quark pair production cross-section. A data sample of 2.05 fb(-1) recorded by the ATLAS detector at the Large Hadron Collider is used. Relative differential cross-sections are derived as a function of the invariant mass, the transverse momentum and the rapidity of the top quark pair system. Events are selected in the lepton (electron or muon) + jets channel. The background-subtracted differential distributions are corrected for detector effects, normalized to the total inclusive top quark pair production cross-section and compared to theoretical predictions. The measurement uncertainties range typically between 10 % and 20 % and are generally dominated by systematic effects. No significant deviations from the Standard Model expectations are observed. C1 [Alam, M. S.; Edson, W.; Ernst, J.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Bahinipati, S.; Chan, K.; Gingrich, D. M.; Moore, R. W.; Pinfold, J. L.; Vaque, F. Vives] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakir, O.; Ciftci, A. K.; Ciftci, R.; Yildiz, H. Duran; Kuday, S.] Ankara Univ, Dept Phys, TR-06100 Ankara, Turkey. Dumlupinar Univ, Dept Phys, Kutahya, Turkey. [Yilmaz, M.] Gazi Univ, Dept Phys, Ankara, Turkey. [Sultansoy, S.] TOBB Univ Econ & Technol, Div Phys, Ankara, Turkey. [Cakir, I. Turk] Turkish Atom Energy Commiss, Ankara, Turkey. [Bella, L. Aperio; Aubert, B.; Berger, N.; Colas, J.; Delmastro, M.; Di Ciaccio, L.; Doan, T. K. O.; Elles, S.; Hryn'ova, T.; Jezequel, S.; Kataoka, M.; Labbe, J.; Lafaye, R.; Leveque, J.; Lombardo, V. P.; Massol, N.; Perrodo, P.; Petit, E.; Przysiezniak, H.; Richter-Was, E.; Sauvage, G.; Sauvan, E.; Schwoerer, M.; Todorov, T.; Tsionou, D.; Wingerter-Seez, I.; Zitoun, R.] CNRS IN2P3, LAPP, Annecy Le Vieux, France. [Bella, L. Aperio; Aubert, B.; Berger, N.; Colas, J.; Delmastro, M.; Di Ciaccio, L.; Doan, T. K. O.; Elles, S.; Hryn'ova, T.; Jezequel, S.; Kataoka, M.; Labbe, J.; Lafaye, R.; Leveque, J.; Lombardo, V. P.; Massol, N.; Perrodo, P.; Petit, E.; Przysiezniak, H.; Richter-Was, E.; Sauvage, G.; Sauvan, E.; Schwoerer, M.; Todorov, T.; Tsionou, D.; Wingerter-Seez, I.; Zitoun, R.] Univ Savoie, Annecy Le Vieux, France. [Asquith, L.; Blair, R. E.; Chekanov, S.; Fellmann, D.; Feng, E. J.; Fernando, W.; Goshaw, A. T.; LeCompte, T.; Malons, D.; Nodulman, L.; Paramonov, A.; Price, L. E.; Proudfoot, J.; Salvachua Ferrando, B. M.; Stanek, R. W.; van Gemmeren, P.; Vaniachine, A.; Yoshida, R.; Zhang, J.] Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. [Cheu, E.; Johns, K. A.; Kaushik, V.; Lampen, C. L.; Lampl, W.; Lei, X.; Loch, P.; Paleari, C. P.; Ruehr, F.; Rutherfoord, J. P.; Shupe, M. A.] Univ Arizona, Dept Phys, Tucson, AZ 85721 USA. [Brandt, A.; Brown, H.; De, K.; Farbin, A.; Heelan, L.; Hernandez, C. M.; Nilsson, P.; Ozturk, N.; Sarkisyan-Grinbaum, E.; Sosebee, M.; Spurlock, B.; Stradling, A. R.; Usai, G.; Vartapetian, A.; White, A.; Yu, J.] Univ Texas Arlington, Dept Phys, Arlington, TX 76019 USA. [Antonaki, A.; Fassouliotis, D.; Giakoumopoulou, V.; Giokaris, N.; Ioannou, P.; Iordanidou, K.; Kourkoumelis, C.; Manousakis-Katsikakis, A.; Tzanakos, G.] Univ Athens, Dept Phys, Athens, Greece. [Alexopoulos, T.; Avramidou, R.; Dris, M.; Gazis, E. N.; Iakovidis, G.; Karakostas, K.; Katsoufis, E.; Leontsinis, S.; Maltezos, S.; Mountricha, E.; Panagiotopoulou, E.; Papadopoulou, Th. D.; Tsipolitis, G.; Vlachos, S.] Natl Tech Univ Athens, Dept Phys, Zografos, Greece. [Abdinov, O.; Khalilzada, F.] Azerbaijan Acad Sci, Inst Phys, Baku 370143, Azerbaijan. [Abdallah, J.; Bosman, M.; Casado, M. P.; Cavalli-Sforza, M.; Conidi, M. C.; Demirkoz, B.; Curull, X. Espinal; Francavilla, P.; Giangiobbe, V.; Gonzalez Parra, G.; Grinstein, S.; Helsens, C.; Rozas, A. Juste; Korolkov, I.; Le Menedeu, E.; Martinez, M.; Mir, L. M.; Montejo Berlingen, J.; Nadal, J.; Osuna, C.; Pages, A. Pacheco; Aranda, C. Padilla; Riu, I.; Rossetti, V.; Rubbo, F.; Succurro, A.; Tsiskaridze, S.; Vorwerk, V.] Univ Autonoma Barcelona, Inst Fis Altes Energies, E-08193 Barcelona, Spain. [Abdallah, J.; Bosman, M.; Casado, M. P.; Cavalli-Sforza, M.; Conidi, M. C.; Demirkoz, B.; Curull, X. Espinal; Francavilla, P.; Giangiobbe, V.; Gonzalez Parra, G.; Grinstein, S.; Helsens, C.; Rozas, A. Juste; Korolkov, I.; Le Menedeu, E.; Martinez, M.; Mir, L. M.; Montejo Berlingen, J.; Nadal, J.; Osuna, C.; Pages, A. Pacheco; Aranda, C. Padilla; Riu, I.; Rossetti, V.; Rubbo, F.; Succurro, A.; Tsiskaridze, S.; Vorwerk, V.] Univ Autonoma Barcelona, Dept Fis, E-08193 Barcelona, Spain. [Abdallah, J.; Bosman, M.; Casado, M. P.; Cavalli-Sforza, M.; Conidi, M. C.; Demirkoz, B.; Curull, X. Espinal; Francavilla, P.; Giangiobbe, V.; Gonzalez Parra, G.; Grinstein, S.; Helsens, C.; Rozas, A. Juste; Korolkov, I.; Le Menedeu, E.; Martinez, M.; Mir, L. M.; Montejo Berlingen, J.; Nadal, J.; Osuna, C.; Pages, A. Pacheco; Aranda, C. Padilla; Riu, I.; Rossetti, V.; Rubbo, F.; Succurro, A.; Tsiskaridze, S.; Vorwerk, V.] ICREA, Barcelona, Spain. [Borjanovic, I.; Krstic, J.; Popovic, D. S.; Sijacki, Dj.; Simic, Lj.] Univ Belgrade, Inst Phys, Belgrade, Serbia. [Bozovic-Jelisavcic, I.; Cirkovic, P.; Jovin, T.; Mamuzic, J.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia. [Buanes, T.; Burgess, T.; Eigen, G.; Kastanas, A.; Liebig, W.; Lipniacka, A.; Rosendahl, P. L.; Sandaker, H.; Sjursen, T. B.; Stugu, B.; Tonoyan, A.; Ugland, M.] Univ Bergen, Dept Phys & Technol, Bergen, Norway. [Arguin, J-F.; Bach, A. M.; Galtieri, A. Barbaro; Barnett, R. M.; Beringer, J.; Biesiada, J.; Calafiura, P.; Caminada, L. M.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Copic, K.; Dube, S.; Einsweiler, K.; Gaponenko, A.; Garcia-Sciveres, M.; Haber, C.; Hance, M.; Heinemann, B.; Hinchliffe, I.; Hsu, S. -C.; Hurwitz, M.; Lavrijsen, W.; Leggett, C.; Loscutoff, P.; Madaras, R. J.; Ovcharova, A.; Griso, S. Pagan; Pranko, A.; Quarrie, D. R.; Ruwiedel, C.; Shapiro, M.; Skinnari, L. A.; Tatarkhanov, M.; Tibbetts, M. J.; Tsulaia, V.; Vahsen, S.; Varouchas, D.; Virzi, J.; Yao, Y.; Zenz, S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Arguin, J-F.; Bach, A. M.; Galtieri, A. Barbaro; Barnett, R. M.; Beringer, J.; Biesiada, J.; Calafiura, P.; Caminada, L. M.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Copic, K.; Dube, S.; Einsweiler, K.; Gaponenko, A.; Garcia-Sciveres, M.; Haber, C.; Hance, M.; Heinemann, B.; Hinchliffe, I.; Hsu, S. -C.; Hurwitz, M.; Lavrijsen, W.; Leggett, C.; Loscutoff, P.; Madaras, R. J.; Ovcharova, A.; Griso, S. Pagan; Pranko, A.; Quarrie, D. R.; Ruwiedel, C.; Shapiro, M.; Skinnari, L. A.; Tatarkhanov, M.; Tibbetts, M. J.; Tsulaia, V.; Vahsen, S.; Varouchas, D.; Virzi, J.; Yao, Y.; Zenz, S.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Aliev, M.; Giorgi, F. M.; Grancagnolo, S.; Herrberg, R.; Hristova, I.; Kind, O.; Kolanoski, H.; Kwee, R.; Lacker, H.; Leyton, M.; Lohse, T.; Mandryschis, R.; Nikiforov, A.; Schulz, H.; Wendland, D.; zur Nedden, M.] Humboldt Univ, Dept Phys, Berlin, Germany. [Agustoni, M.; Ancu, L. S.; Battaglia, A.; Beck, H. P.; Borer, C.; Ereditato, A.; Martin, T. Fonseca; Gallo, V.; Haug, S.; Kabana, S.; Kruker, T.; Marti, L. F.; Pretzl, K.; Schneider, B.; Topfel, C.; Weber, M. S.] Univ Bern, Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Agustoni, M.; Ancu, L. S.; Battaglia, A.; Beck, H. P.; Borer, C.; Ereditato, A.; Martin, T. Fonseca; Gallo, V.; Haug, S.; Kabana, S.; Kruker, T.; Marti, L. F.; Pretzl, K.; Schneider, B.; Topfel, C.; Weber, M. S.] Univ Bern, High Energy Phys Lab, Bern, Switzerland. [Allbrooke, B. M. M.; Bansil, H. S.; Bracinik, J.; Charlton, D. G.; Chisholm, A. S.; Collins, N. J.; Curtis, C. J.; Garvey, J.; Hadley, D. R.; Hawkes, C. M.; Head, S. J.; Hillier, S. J.; Mahout, G.; Martin's, T. A.; Mclaughlan, T.; Newman, P. R.; Nikolopoulos, K.; O'Neale, S. W.; Palmer, J. D.; Slater, M.; Thomas, J. P.; Thompson, P. D.; Watkins, P. M.; Watson, A. T.; Wilson, J. A.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Akdogan, T.; Arik, E.; Arik, M.; Istin, S.; Ozcan, V. E.; Rador, T.] Bogazici Univ, Dept Phys, Istanbul, Turkey. [Cetin, S. A.] Dogus Univ, Div Phys, Istanbul, Turkey. [Beddall, A. J.; Beddall, A.; Bingul, A.] Gaziantep Univ, Dept Phys Engn, Gaziantep, Turkey. Istanbul Tech Univ, Dept Phys, TR-80626 Istanbul, Turkey. [Bellagamba, L.; Bertin, A.; Bindi, M.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; Caforio, D.; Ciocca, C.; Corradi, M.; De Castro, S.; Di Sipio, R.; Fabbri, L.; Franchini, M.; Giacobbe, B.; Giusti, P.; Grafstroem, P.; Jha, M. K.; Massa, I.; Mengarelli, A.; Monzani, S.; Negrini, M.; Piccinini, M.; Polini, A.; Rinaldi, L.; Romano, M.; Sbarra, C.; Sbrizzi, A.; Semprini-Cesari, N.; Spighi, R.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Bertin, A.; Bindi, M.; Caforio, D.; Ciocca, C.; De Castro, S.; Di Sipio, R.; Fabbri, L.; Franchini, M.; Grafstroem, P.; Massa, I.; Mengarelli, A.; Monzani, S.; Piccinini, M.; Romano, M.; Sbrizzi, A.; Semprini-Cesari, N.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, Dipartmento Fis, Bologna, Italy. [Abajyan, T.; Arutinov, D.; Backhaus, M.; Barbero, M.; Bechtle, P.; Brock, I.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Gaycken, G.; Geich-Gimbel, Ch.; Gonella, L.; Haefner, P.; Havranek, M.; Hellmich, D.; Hillert, S.; Huegging, F.; Ince, T.; Karagounis, M.; Khoriauli, G.; Koevesarki, P.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lapoire, C.; Lehmacher, M.; Leyko, A. M.; Limbach, C.; Loddenkoetter, T.; Mazur, M.; Moeser, N.; Mueller, K.; Nanava, G.; Nattermann, T.; Nuncio-Quiroz, A. -E.; Psoroulas, S.; Schaepe, S.; Schmieden, K.; Schmitz, M.; Schultens, M. J.; Schwindt, T.; Stillings, J. A.; Therhaag, J.; Tsung, J. -W.; Uchida, K.; Uhlenbrock, M.; Vogel, A.; von Toerne, E.; Wang, T.; Wermes, N.; Wienemann, P.; Zendler, C.; Zimmermann, R.; Zimmermann, S.] Univ Bonn, Inst Phys, Bonn, Germany. [Ahlen, S. P.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Love, J.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, Boston, MA 02215 USA. [Aefsky, S.; Amelung, C.; Bensinger, J. R.; Blocker, C.; Daya-Ishmukhametova, R. K.; Pomeroy, D.; Sciolla, G.; Wellenstein, H.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Perantoni, M.; Seixas, J. M.] Univ Fed Rio De Janeiro COPPE EE IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; Manhaes de Andrade Filho, L.] Univ Fed Juiz de Fora, Juiz de Fora, Brazil. [do Vale, M. A. B.] Univ Fed Sao Joao del Rei, Sao Joao del Rei, Brazil. [Donadelli, M.; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Ahmad, A.; Assamagan, K.; Baker, M. D.; Begel, M.; Bernius, C.; Chen, H.; Chernyatin, V.; Debbe, R.; Dhullipudi, R.; Ernst, M.; Gadfort, T.; Gibbard, B.; Gordon, H. A.; Greenwood, Z. D.; Klimentov, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Majewski, S.; Nevski, P.; Okawa, H.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Park, W.; Pleier, M-A.; Poblaguev, A.; Polychronakos, V.; Pravahan, R.; Protopopescu, S.; Purohit, M.; Rahm, D.; Rajagopalan, S.; Redlinger, G.; Sawyer, L.; Sircar, A.; Snyder, S.; Steinberg, P.; Stumer, I.; Takai, H.; Tamsett, M. C.; Triplett, N.; Undrus, A.; Wenaus, T.; Ye, S.; Yu, D.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Badescu, E.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Cuciuc, C. -M.; Dinut, F.; Dita, P.; Dita, S.; Micu, L.; Olariu, A.; Pantea, D.; Popeneciu, G. A.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Darlea, G. L.] Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Gonzalez Silva, M. L.; Otero y Garzon, G.; Piegaia, R.; Romeo, G.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Ask, S.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Buttinger, W.; Carter, J. R.; Chapman, J. D.; Cowden, C.; French, S. T.; Frost, J. A.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Moeller, V.; Parker, M. A.; Robinson, D.; Sandoval, T.; Thomson, M.; Ward, C. P.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Gillberg, D.; Koffas, T.; Liu, C.; Marchand, J. F.; McCarthy, T. G.; Oakham, F. G.; Randrianarivony, K.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Anastopoulos, C.; Anghinolfi, F.; Baak, M. A.; Bachas, K.; Banfi, D.; Battistin, M.; Bellina, F.; Bellomo, M.; Beltramello, O.; Berge, D.; Bianchi, R. M.; Blanchot, G.; Bogaerts, J. A.; Boyd, J.; Bremer, J.; Burckhart, H.; Byszewski, M.; Campana, S.; Capeans Garrido, M. D. M.; Carli, T.; Catmore, J. R.; Cattai, A.; Cerri, A.; Chavez Barajas, C. A.; Childers, J. T.; Chromek-Burckhart, D.; Cote, D.; Danielsson, H. O.; Dell'Acqua, A.; Di Girolamo, A.; Di Girolamo, B.; Di Micco, B.; Dittus, F.; Dobinson, R.; Dobos, D.; Dobson, E.; Dopke, J.; Dudarev, A.; Duehrssen, M.; Dunford, M.; Dydak, F.; Ellis, N.; Elsing, M.; Fabre, C.; Farthouat, P.; Fassnacht, P.; Francis, D.; Franz, S.; Froeschl, R.; Froidevaux, D.; Torregrosa, E. Fullana; Gabaldon, C.; Garelli, N.; Garonne, V.; Gianotti, F.; Gibson, S. M.; Godlewski, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Haas, S.; Hahn, F.; Haider, S.; Hauschild, M.; Hawkings, R. J.; Heller, M.; Henriques Correia, A. M.; Hervas, L.; Hoecker, A.; Huhtinen, M.; Inigo-Golfin, J.; Jaekel, M. R.; Jansen, H.; Jenni, P.; Joram, C.; Jungst, R. M.; Kaneda, M.; Kaplon, J.; Kerschen, N.; Klioutchnikova, T.; Koeneke, K.; Lamanna, M.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Magnoni, L.; Malaescu, B.; Malyukov, S.; Mapelli, A.; Mapelli, L.; Marshall, Z.; Martin, B.; Messina, A.; Meyer, T. C.; Michal, S.; Morley, A. K.; Mornacchi, G.; Muenstermann, D.; Nairz, A. M.; Nakahama, Y.; Negri, G.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Ohm, C. C.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Petersen, J.; Piacquadio, G.; Pommes, K.; Poppleton, A.; Portell Bueso, X.; Poulard, G.; Prasad, S.; Raymond, M.; Rembser, C.; Roda Dos Santos, D.; Roe, S.; Salek, D.; Salzburger, A.; Savu, D. O.; Schlenker, S.; Schott, M.; Sfyrla, A.; Shimizu, S.; Spigo, G.; Spiwoks, R.; Stewart, G. A.; Ten Kate, H.; Torchiani, I.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van der Ster, D.; van Eldik, N.; Vandelli, W.; Veness, R.; Vinek, E.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Winklmeier, F.; Wotschack, J.; Zajacova, Z.; Zwalinski, L.] CERN, Geneva, Switzerland. [Anderson, K. J.; Boveia, A.; Canelli, F.; Choudalakis, G.; Costin, T.; Fiascaris, M.; Gardner, R. W.; Plante, I. Jen-La; Kapliy, A.; Melachrinos, C.; Merritt, F. S.; Meyer, C.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Shochet, M. J.; Tompkins, L.; Tuggle, J. M.; Vukotic, I.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Diaz, M. A.; Olivares Pino, S. A.; Quinonez, F.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Carquin, E.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Jin, S.; Lu, F.; Ouyang, Q.; Ruan, X.; Shan, L. Y.; Yao, L.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Han, L.; Jiang, Y.; Li, S.; Liu, M.; Liu, Y.; Peng, H.; Wang, H.; Wu, Y.; Xu, C.; Zhang, D.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Feng, C.; Ge, P.; He, M.; Miao, J.; Zhan, Z.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Toro, R. Camacho; Cinca, D.; Donini, J.; Febbraro, R.; Ghodbane, N.; Guicheney, C.; Liao, H.; Pallin, D.; Paredes Hernandez, D.; Podlyski, F.; Santoni, C.; Vazeille, F.] Clermont Univ, Phys Corpusculaire Lab, Aubiere, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Toro, R. Camacho; Cinca, D.; Donini, J.; Febbraro, R.; Ghodbane, N.; Guicheney, C.; Liao, H.; Pallin, D.; Paredes Hernandez, D.; Podlyski, F.; Santoni, C.; Vazeille, F.] Univ Clermont Ferrand, Aubiere, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Toro, R. Camacho; Cinca, D.; Donini, J.; Febbraro, R.; Ghodbane, N.; Guicheney, C.; Liao, H.; Pallin, D.; Paredes Hernandez, D.; Podlyski, F.; Santoni, C.; Vazeille, F.] CNRS IN2P3, Aubiere, France. [Andeen, T.; Angerami, A.; Brooijmans, G.; Chen, Y.; Dodd, J.; Grau, N.; Guo, J.; Hughes, E. W.; Nikiforou, N.; Parsons, J. A.; Penson, A.; Perez, K.; Perez Reale, V.; Scherzer, M. I.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Williams, E.; Willis, W.; Wulf, E.; Zivkovic, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Boelaert, N.; Dam, M.; Gregersen, K.; Hansen, J. R.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Heisterkamp, S.; Jakobsen, S.; Jez, P.; Joergensen, M. D.; Kadlecik, P.; Klinkby, E. B.; Lundquist, J.; Mackeprang, R.; Mehlhase, S.; Petersen, T. C.; Simonyan, M.; Thomsen, L. A.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; Fazio, S.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Morello, G.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, INFN Grp Coll Cosenza, Arcavacata Di Rende, Italy. [Capua, M.; Crosetti, G.; Fazio, S.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Morello, G.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Banas, E.; Blocki, J.; Bruckman de Renstrom, P. A.; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Malecki, P.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Turala, M.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.; Zemla, A.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Yagci, K. Dindar; Firan, A.; Hadavand, H. K.; Hoffman, J.; Ishmukhametov, R.; Joffe, D.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Rios, R. R.; Sekula, S. J.; Stroynowski, R.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Ahsan, M.; Izen, J. M.; Lou, X.; Reeves, K.; Wong, W. C.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Kuutmann, E. Bergeaas; Dassoulas, J. A.; Dietrich, J.; Ehrenfeld, W.; Ferrara, V.; Fischer, G.; Friedrich, C.; Glazov, A.; Goebel, M.; Gomez Fajardo, L. S.; Firmino Da Costa, J. Goncalves Pinto; Gosdzik, B.; Grahn, K-J.; Gregor, I. M.; Hiller, K. H.; Huettmann, A.; Husemann, U.; Jimenez Belenguer, M.; Johnert, S.; Karnevskiy, M.; Katzy, J.; Kono, T.; Kuhl, T.; Lange, C.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Perez Cavalcanti, T.; Petschull, D.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Stanescu-Bellu, M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Zhu, H.] DESY, Hamburg, Germany. [Kuutmann, E. Bergeaas; Dassoulas, J. A.; Dietrich, J.; Ehrenfeld, W.; Ferrara, V.; Fischer, G.; Friedrich, C.; Glazov, A.; Goebel, M.; Gomez Fajardo, L. S.; Firmino Da Costa, J. Goncalves Pinto; Gosdzik, B.; Grahn, K-J.; Gregor, I. M.; Hiller, K. H.; Huettmann, A.; Husemann, U.; Jimenez Belenguer, M.; Johnert, S.; Karnevskiy, M.; Katzy, J.; Kono, T.; Kuhl, T.; Lange, C.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Perez Cavalcanti, T.; Petschull, D.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Stanescu-Bellu, M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Zhu, H.] DESY, Zeuthen, Germany. [Bunse, M.; Esch, H.; Goessling, C.; Hirsch, F.; Jung, C. A.; Klingenberg, R.; Reisinger, I.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Czodrowski, P.; Friedrich, F.; Goepfert, T.; Kobel, M.; Leonhardt, K.; Ludwig, A.; Mader, W. F.; Morgenstern, M.; Prudent, X.; Rudolph, C.; Schnoor, U.; Schwierz, R.; Seifert, F.; Steinbach, P.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Ko, B. R.; Kotwal, A.; Oh, S. H.; Wang, C.; Yamaoka, J.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Buckley, A. G.; Clark, P. J.; Debenedetti, C.; Harrington, R. D.; Martin, V. J.; O'Brien, B. J.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Cerutti, F.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.; Volpi, G.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Aad, G.; Ahles, F.; Barber, T.; Bernhard, R.; Bitenc, U.; Boehler, M.; Bruneliere, R.; Christov, A.; Consorti, V.; Fehling-Kaschek, M.; Flechl, M.; Glatzer, J.; Hartert, J.; Herten, G.; Horner, S.; Jakobs, K.; Janus, M.; Kollefrath, M.; Kononov, A. I.; Kuehn, S.; Lai, S.; Landgraf, U.; Lohwasser, K.; Ludwig, I.; Ludwig, J.; Lumb, D.; Mahboubi, K.; Mohr, W.; Nilsen, H.; Parzefall, U.; Rammensee, M.; Rave, T. C.; Rurikova, Z.; Schmidt, E.; Schumacher, M.; Siegert, F.; Stoerig, K.; Sundermann, J. E.; Temming, K. K.; Thoma, S.; Tsiskaridze, V.; Venturi, M.; Vivarelli, I.; von Radziewski, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Wiik-Fuchs, L. A. M.; Winkelmann, S.; Xie, S.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Abdelalim, A. A.; Alexandre, G.; Backes, M.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; Blondel, A.; Bucci, F.; Clark, A.; Dao, V.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Iacobucci, G.; La Rosa, A.; Lister, A.; Latour, B. Martin Dit; Mermod, P.; Mora Herrera, C.; Nektarijevic, S.; Nikolics, K.; Pasztor, G.; Picazio, A.; Pohl, M.; Rosbach, K.; Rosselet, L.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Beccherle, R.; Caso, C.; Dameri, M.; Darbo, G.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Barberis, D.; Caso, C.; Dameri, M.; Parodi, A. Ferretto; Gagliardi, G.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Chikovani, L.; Tskhadadzea, E. G.] Tbilisi State Univ, E Andronikashvili Inst Phys, GE-380086 Tbilisi, Rep of Georgia. [Djobava, T.; Khubua, J.; Mchedlidze, G.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Bussey, P.; Buttar, C. M.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Edwards, N. C.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Kar, D.; Kenyon, M.; Moraess, A.; O'Shea, V.; Oropeza Barrera, C.; Robson, A.; Saxon, D. H.; Smith, K. M.; St Denis, R. D.; Steele, G.; Thompson, A. S.; Wraight, K.; Wright, C.; Wright, M.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bierwagen, K.; Blumenschein, U.; Brandt, O.; Catastini, P.; Erdmann, J.; Evangelakou, D.; George, M.; Grosse-Knetter, J.; Guindon, S.; Haller, J.; Hamer, M.; Henrichs, A.; Hensel, C.; Keil, M.; Knue, A.; Kohn, F.; Krieger, N.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Mann, A.; Meyer, J.; Morel, J.; Pashapour, S.; Quadt, A.; Roe, A.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Uhrmacher, M.; Schroeder, T. Vazquez; Weber, P.; Weingarten, J.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Maleka, F.; Stark, J.; Sun, X.; Trocme, B.; Wang, J.; Weydert, C.] Univ Grenoble 1, Lab Phys Subat & Cosmol, Grenoble, France. [Albrand, S.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Maleka, F.; Stark, J.; Sun, X.; Trocme, B.; Wang, J.; Weydert, C.] CNRSIN2P3, Grenoble, France. [Albrand, S.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Maleka, F.; Stark, J.; Sun, X.; Trocme, B.; Wang, J.; Weydert, C.] Inst Natl Polytech Grenoble, F-38031 Grenoble, France. [Addy, T. N.; Harvey, A.; McFarlane, K. W.; Shin, T.; Vassilakopoulos, V. I.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Guimaraes da Costa, J. Barreiro; Belloni, A.; Conti, G.; Huth, J.; Jeanty, L.; Kagan, M.; Mateos, D. Lopez; Mercurio, K. M.; Mills, C.; Morii, M.; Skottowe, H. P.; Smith, B. C.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Davygora, Y.; Dietzsch, T. A.; Geweniger, C.; Hanke, P.; Henke, M.; Khomich, A.; Kluge, E. -E.; Lang, V. S.; Lendermann, V.; Lepold, F.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Anders, G.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Kugel, A.; Maenner, R.; Schroer, N.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Cwetanski, P.; Evans, H.; Gagnon, P.; Jain, V.; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Price, D.; Whittington, D.; Yang, Y.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Epp, B.; Jussel, P.; Kneringer, E.; Kuhn, D.; Lukas, W.; Rudolph, G.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Limper, M.; Mallik', U.; Pylypchenko, Y.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Meyer, W. T.; Prell, S.; Rosenberg, E. I.; Ruiz-Martinez, A.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Aleksandrov, I. N.; Bardin, D. Y.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Dova, M. T.; Glonti, G. L.; Gostkin, M. I.; Grigalashvili, N.; Huseynov, N.; Kalinovskaya, L. V.; Kazarinov, M. Y.; Kekelidze, G. D.; Kharchenko, D.; Khramov, E.; Kolesnikov, V.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Pozdnyakov, V.; Rumyantsev, L.; Rusakovich, N. A.; Sadykov, R.; Shiyakova, M.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.; Zimin, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Arai, Y.; Doi, Y.; Haruyama, T.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Makida, Y.; Manabe, A.; Mitsui, S.; Nagano, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Hayakawa, T.; King, M.; Kishimoto, T.; Kitamura, T.; Kurashige, H.; Matsushita, T.; Ochi, A.; Suzuki, Y.; Takeda, H.; Tani, K.; Watanabe, I.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Sasao, N.; Sumida, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto, Japan. [Kawagoe, K.; Oda, S.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alonso, F.; Anduaga, X. S.; Monticelli, F.; Tripiana, M. F.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Alonso, F.; Anduaga, X. S.; Monticelli, F.; Tripiana, M. F.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Davidson, R.; de Mora, L.; Dearnaley, W. J.; Fox, H.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Bianco, M.; Cataldi, G.; Chiodini, G.; Gorini, E.; Grancagnolo, F.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Bianco, M.; Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; Cindro, V.; D'Onofrio, M.; Dervan, P.; Greenshaw, T.; Gwilliam, C. B.; Hayward, H. S.; Jackson, J. N.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kluge, T.; Kretzschmar, J.; Laycock, P.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Sellers, G.; Vossebeld, J. H.; Waller, P.; Wrona, B.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Deliyergiyev, M.; Dolenc, I.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Deliyergiyev, M.; Dolenc, I.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia. [Adragna, P.; Bona, M.; Carter, A. A.; Cerrito, L.; Ellis, K.; Goddard, J. R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Poll, J.; Rizvi, E.; Salamanna, G.; Teixeira Dias Castanheira, M.; Wiglesworth, C.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Alam, M. A.; Berry, T.; Boisvert, V.; Brooks, T.; Cantrill, R.; Cowan, G.; Duguid, L.; Edwards, C. A.; Eisenhandler, E.; George, S.; Gonalo, R.; Hayden, D.; Pastore, Fr.; Rose, M.; Spano, F.; Strong, J. A.; Teixeira-Dias, P.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Baker, S.; Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Chislett, R. T.; Christidi, I. A.; Cooper, B. D.; Davison, A. R.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Kramberger, G.; Lambourne, L.; Monk, J.; Nash, M.; Nurse, E.; Prabhu, R.; Sherwood, P.; Simmons, B.; Taylor, C.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Cavalleri, P.; Chareyre, E.; Davignon, O.; De Cecco, S.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph.; Theveneaux-Pelzer, T.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Cavalleri, P.; Chareyre, E.; Davignon, O.; De Cecco, S.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph.; Theveneaux-Pelzer, T.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Cavalleri, P.; Chareyre, E.; Davignon, O.; De Cecco, S.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph.; Theveneaux-Pelzer, T.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] CNRS IN2P3, Paris, France. [Akesson, T. P. A.; Alonso, A.; Bocchetta, S. S.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Jarlskog, G.; Lundberg, B.; Lytken, E.; Meirose, B.; Mjoernmark, J. U.; Smirnova, O.] Lund Univ, Fysiska Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Labarga, L.; Lagouri, T.; Merino, J. Llorente; March, L.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Aharrouche, M.; Arnaez, O.; Blum, W.; Buescher, V.; Caputo, R.; Eckweiler, S.; Edmonds, K.; Ellinghaus, F.; Ertel, E.; Fiedler, F.; Fleckner, J.; Goeringer, C.; Handel, C.; Hohlfeld, M.; Hsu, P. J.; Ji, W.; Kawamura, G.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lungwitz, M.; Masetti, L.; Meyer, C.; Moreno, D.; Mueller, T.; Neusiedl, A.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schroeder, C.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Almond, J.; Borri, M.; Brown, G.; Chavda, V.; Cox, B. E.; Da Via, C.; Duerdoth, I. P.; Forti, A.; Howarth, J.; Ibbotson, M.; Joshi, K. D.; Klinger, J. A.; Lane, J. L.; Loebinger, F. K.; Marx, M.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Pilkington, A. D.; Robinson, J. E. M.; Schwanenberger, C.; Snow, S. W.; Watts, S.; Woudstra, M. J.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aoun, S.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Odier, J.; Pralavorio, P.; Rozanov, A.; Talby, M.; Tannoury, N.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aoun, S.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Odier, J.; Pralavorio, P.; Rozanov, A.; Talby, M.; Tannoury, N.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] CNRS IN2P3, Marseille, France. [Brau, B.; Colon, G.; Dallapiccola, C.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Caron, B.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Dobbs, M.; Dufour, M-A.; Guler, H.; Klemetti, M.; Robertson, S. H.; Santamarina Rios, C.; Schram, M.; Stockton, M. C.; Vachon, B.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Davidson, N.; Diglio, S.; Jennens, D.; Kubota, T.; Limosani, A.; Moorhead, G. F.; Hanninger, G. Nunes; Phan, A.; Shao, Q. T.; Soni, N.; Taylor, G. N.; Thong, W. M.; Volpi, M.; White, M. J.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Armbruster, A. J.; Borroni, S.; Chapman, J. W.; Cirilli, M.; Dai, T.; Diehl, E. B.; Ferretti, C.; Goldfarb, S.; Harper, D.; Levin, D.; Li, X.; Liu, H.; Liu, J. B.; Liu, L.; Mc Kee, S. P.; Neal, H. A.; Panikashvili, N.; Purdham, J.; Qian, J.; Scheirich, D.; Thun, R. P.; Walch, S.; Wilson, A.; Wooden, G.; Yang, H.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Alvarez Gonzalez, B.; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Fedorko, W.; Hauser, R.; Heim, S.; Holzbauer, J. L.; Huston, J.; Koll, J.; Linnemann, J. T.; Mangeard, P. S.; Martin, B.; Miller, R. J.; Pope, B. G.; Ryan, P.; Schwienhorst, R.; Stelzer, H. J.; Tollefson, K.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Acerbi, E.; Alessandria, F.; Alimonti, G.; Andreazza, A.; Baccaglioni, G.; Besana, M. I.; Broggi, F.; Carminati, L.; Cavalli, D.; Citterio, M.; Consonni, S. M.; Costa, G.; Fanti, M.; Favareto, A.; Giugni, D.; Koletsou, I.; Lari, T.; Mandelli, L.; Mazzanti, M.; Meloni, F.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Rivoltella, G.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Vegni, G.; Volpini, G.] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Acerbi, E.; Andreazza, A.; Besana, M. I.; Carminati, L.; Consonni, S. M.; Fanti, M.; Favareto, A.; Meloni, F.; Perini, L.; Pizio, C.; Ragusa, F.; Rivoltella, G.; Simoniello, R.; Turra, R.; Vegni, G.] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Satsounkevitch, I.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Azuelos, G.; Banerjee, P.; Bouchami, J.; Davies, M.; Giunta, M.; Leroy, C.; Martin, J. P.; Mehdiyev, R.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Sulin, V. V.; Tikhomirov, V. O.] Acad Sci, PN Lebedev Inst Phys, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] ITEP, Moscow, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.] MEPhI, Moscow, Russia. [Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Snesarev, A. A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Akimov, A. V.; Beale, S.; Becker, S.; Biebel, O.; Calfayan, P.; de Graat, J.; Duckeck, G.; Ebke, J.; Elmsheuser, J.; Engl, A.; Galea, C.; Heller, C.; Hertenberger, R.; Kummer, C.; Legger, F.; Lichtnecker, M.; Lorenz, J.; Mameghani, R.; Mueller, T. A.; Nunnemann, T.; Oakes, L. B.; Rauscher, F.; Reznicek, P.; Ruckert, B.; Sanders, M. P.; Schaile, D.; Schieck, J.; Serfon, C.; Staude, A.; Vladoiu, D.; Walker, R.; Zhuang, X.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Beimforde, M.; Bethke, S.; Bronner, J.; Capriotti, D.; Cortiana, G.; Dubbert, J.; Flowerdew, M. J.; Giovannini, P.; Jantsch, A.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kotov, S.; Kroha, H.; Macchiolo, A.; Menke, S.; Moser, H. G.; Nagel, M.; Nisius, R.; Oberlack, H.; Pahl, C.; Pospelov, G. E.; Potrap, I. N.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Seuster, R.; Stern, S.; Stonjek, S.; Vanadia, M.; von der Schmitt, H.; von Loeben, J.; Weigell, P.; Zhuravlov, V.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Capasso, L.; Carlino, G.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; della Volpe, D.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Musto, E.; Patricelli, S.; Sanchez, A.; Sekhniaidze, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Capasso, L.; Chiefari, G.; della Volpe, D.; Giordano, R.; Merola, L.; Musto, E.; Patricelli, S.; Sanchez, A.] Univ Naples Federico II, Dipartimento Sci Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Metcalfe, J.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Chelstowska, M. A.; De Groot, N.; Filthaut, F.; Klok, P. F.; Koenig, A. C.; Koetsveld, F.; Raas, M.; Salvucci, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Doxiadis, A. D.; Ferrari, P.; Garitaonandia, H.; Geerts, D. A. A.; Gosselink, M.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kayl, M. S.; Klous, S.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Luijckx, G.; Massaro, G.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Pani, P.; Rijpstra, M.; Ruckstuhl, N.; Ta, D.; Tsiakiris, M.; Turlay, E.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van der Kraaij, E.; Van der Leeuw, R.; van der Poel, E.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Doxiadis, A. D.; Ferrari, P.; Garitaonandia, H.; Geerts, D. A. A.; Gosselink, M.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kayl, M. S.; Klous, S.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Luijckx, G.; Massaro, G.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Pani, P.; Rijpstra, M.; Ruckstuhl, N.; Ta, D.; Tsiakiris, M.; Turlay, E.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van der Kraaij, E.; Van der Leeuw, R.; van der Poel, E.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.] Univ Amsterdam, Amsterdam, Netherlands. [Calkins, R.; Chakraborty, D.; Cole, S.; Rocha de Lima, J. G.; Suhr, C.; Yurkewicz, A.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A.; Beloborodova, O.; Bobrovnikov, V. B.; Bogdanchikov, A.; Kazanin, V. A.; Kolachev, G. M.; Korol, A.; Malyshevm, V.; Maslennikov, A. L.; Orlov, I.; Peleganchuk, S. V.; Schamov, A. G.; Skovpen, K.; Soukharev, A.; Talyshev, A.; Tikhonov, Y. A.; Zaytsev, A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Budick, B.; Casadei, D.; Cranmer, K.; van Huysduynen, L. Hooft; Konoplich, R.; Krasznahorkay, A.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethym, P.; Neves, R. M.; Prokofiev, K.; Shibata, A.; Zhao, L.] NYU, Dept Phys, New York, NY 10003 USA. [Fisher, M. J.; Gan, K. K.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Rahimi, A. M.; Strang, M.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Gutierrez, P.; Jana, D. K.; Marzin, A.; Meera-Lebbai, R.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Snow, J.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Khanov, A.; Rizatdinova, F.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Hamal, P.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Potter, C. T.; Ptacek, E.; Radloff, P.; Reinsch, A.; Searcy, J.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Andari, N.; Arnault, C.; Auge, E.; Barrillon, P.; Benoit, M.; Binet, S.; Bourdarios, C.; De La Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Matricon, P.; Niedercorn, F.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Teinturier, M.; Veillet, J. J.; Wicek, F.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Andari, N.; Arnault, C.; Auge, E.; Barrillon, P.; Benoit, M.; Binet, S.; Bourdarios, C.; De La Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Matricon, P.; Niedercorn, F.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Teinturier, M.; Veillet, J. J.; Wicek, F.; Zerwas, D.; Zhang, Z.] CNRS IN2P3, Orsay, France. [Hanagaki, K.; Hirose, M.; Lee, J. S. H.; Meguro, T.; Nomachi, M.; Sugaya, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Buran, T.; Cameron, D.; Gjelsten, B. K.; Lund, E.; Ould-Saada, F.; Pajchel, K.; Read, A. L.; Rohne, O.; Samset, B. H.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Apolle, R.; Barr, A. J.; Boddy, C. R.; Brandt, G.; Buchanan, J.; Buckingham, R. M.; Coniavitis, E.; Cooper-Sarkar, A. M.; Dafinca, A.; Davies, E.; Gallas, E. J.; Gwenlan, C.; Hall, D.; Hays, C. P.; Howard, J.; Huffman, T. B.; Issever, C.; King, R. S. B.; Kogan, L. A.; Korn, A.; Larner, A.; Lewis, A.; Liang, Z.; Livermore, S. S. A.; Mattravers, C.; Nickerson, R. B.; Pinder, A.; Robichaud-Veronneau, A.; Ryder, N. C.; Short, D.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Whitehead, S. R.; Young, C. J.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Colombo, T.; Conta, C.; Ferrari, R.; Franchino, S.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Uslenghi, M.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Colombo, T.; Conta, C.; Franchino, S.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.; Uslenghi, M.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Brendlinger, K.; Degenhardt, J.; Fratina, S.; Hines, E.; Hong, T. M.; Jackson, B.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Olivito, D.; Ospanov, R.; Reece, R.; Saxon, J.; Schaefer, D.; Stahlmann, J.; Thomson, E.; Wagner, P.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Maleev, V. P., I; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Bertolucci, F.; Cascella, M.; Cavasinni, V.; Crescioli, F.; Del Prete, T.; Dotti, A.; Roda, C.; Sarri, F.; White, S.; Zinonos, Z.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Bertolucci, F.; Cascella, M.; Cavasinni, V.; Crescioli, F.; Del Prete, T.; Dotti, A.; Roda, C.; Sarri, F.; White, S.; Zinonos, Z.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Boudreau, J.; Cleland, W.; Escobar, C.; Kittelmann, T.; Mueller, J.; Prieur, D.; Savinov, V.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Amorim, A.; Anjos, N.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; De Sousa, M. J. Da Cunha Sargedas; Wemans, A. Do Valle; Fiolhais, M. C. N.; Gomes, A.; Jorge, P. M.; Lopes, L.; Miguens, J. Machado; Maio, A.; Maneira, J.; Oliveira, M.; Onofre, A.; Palma, A.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. [Bohm, J.; Chudoba, J.; Gallus, P.; Gunther, J.; Jakoubek, T.; Juranek, V.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Marcisovsky, M.; Mikestikova, M.; Myska, M.; Nemecek, S.; Ruzicka, P.; Schovancova, J.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Tic, T.; Valenta, J.; Vrba, V.; Zeman, M.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Kodys, P.; Leitner, R.; Novakova, J.; Rybar, M.; Spousta, M.; Strachota, P.; Suk, M.; Sykora, T.; Tas, P.; Valkar, S.; Vorobel, V.; Wilhelm, I.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Augsten, K.; Holy, T.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Kral, V.; Krejci, F.; Pospisil, S.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solar, M.; Solc, J.; Sopko, V.; Sopko, B.; Stekl, I.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.] Czech Tech Univ, Prague, Czech Republic. [Ammosov, V. V.; Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Ivashin, A. V.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.; Zmouchko, V. V.] State Res Ctr Inst High Energy Phys, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Gillman, A. R.; Haywood, S. J.; Kirk, J.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Norton, P. R.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Strube, J.; Tyndel, M.; Weber, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Benslama, K.; Smit, G. V. Ybeles] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Artoni, G.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Pedis, D.; De Salvo, A.; De Zorzi, G.; Dionisi, C.; Falciano, S.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Rossi, E.; Tehrani, F. Safai; Sidoti, A.; Camillocci, E. Solfaroli; Vari, R.; Veneziano, S.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma 1, Rome, Italy. [Artoni, G.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Zorzi, G.; Dionisi, C.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Rossi, E.; Camillocci, E. Solfaroli; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Di Simone, A.; Liberti, B.; Marchese, F.; Mazzaferro, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Cattani, G.; Di Ciaccio, A.; Di Simone, A.; Marchese, F.; Mazzaferro, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Branchini, P.; Ceradini, F.; Di Luise, S.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Stanescu, C.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Luise, S.; Orestano, D.; Pastore, F.; Petrucci, F.] Univ Roma Tre, Dipartimento Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.; Lablak, S.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA, Fac Sci Semlalia, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Cherkaoui El Moursli, R.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Abreu, H.; Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Bolnet, N. M.; Boonekamp, M.; Chevalier, L.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Gauthier, L.; Giraud, P. F.; Guyot, C.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Legendre, M.; Maiani, C.; Mal, P.; Manjarres Ramos, J. A.; Mansoulie, B.; Meyer, J-P.; Mijovic, L.; Morange, N.; Hong, V. Nguyen Thi; Nicolaidou, R.; Ouraou, A.; Resende, B.; Royon, C. R.; Schune, Ph.; Schwindling, J.; Simard, O.; Virchaux, M.; Vranjes, N.; Xiao, M.] CEA Saclay, DSM, IRFU, Gif Sur Yvette, France. [Chouridou, S.; Damiani, D. S.; Grillo, A. A.; Hare, G. A.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Mitrevski, J.; Nielsen, J.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Beckingham, M.; Coccaro, A.; Goussiou, A. G.; Griffiths, J.; Harris, O. M.; Keller, J. S.; Lubatti, H. J.; Rothberg, J.; Verducci, M.; Watts, G.; Zhao, T.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Booth, C. N.; Costanzo, D.; Cuhadar Donszelmann, T.; Dawson, I.; Duxfield, R.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Mayne, A.; Mcfayden, J. A.; Miyagawa, P. S.; Owen, S.; Paganis, E.; Suruliz, K.; Tovey, D. R.; Tua, A.; Xu, D.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Holder, M.; Ibragimov, I.; Rammes, M.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Dawe, E.; Godfrey, J.; Kvita, J.; O'Neil, D. C.; Petteni, M.; Stelzer, B.; Tanasijczuk, A. J.; Trottier-McDonald, M.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Butler, B.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Grenier, P.; Haas, A.; Hansson, P.; Horn, C.; Jackson, P.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nelson, T. K.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Smith, D.; Strauss, E.; Su, D.; Wilson, M. G.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Batkova, L.; Blazek, T.; Federic, P.; Pecsy, M.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Ferencei, J.; Kladiva, E.; Seman, M.; Strizenec, P.] Slovak Acad Sci, Dept Subnucl Phys, Inst Expt Phys, Kosice, Slovakia. [Aurousseau, M.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Hamilton, A.; Leney, K. J. C.; Vickey, T.; Vickey Boeriu, O. E.; Yacoob, S.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Asman, B.; Bendtz, K.; Bohm, C.; Clement, C.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Holmgren, S. O.; Johansen, M.; Johansson, K. E.; Jon-And, K.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Papadelis, A.; Sellden, B.; Silverstein, S. B.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Asman, B.; Bendtz, K.; Clement, C.; Gellerstedt, K.; Hellman, S.; Johansen, M.; Jon-And, K.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Ahmad, A.; Arfaoui, S.; Devetak, E.; DeWilde, B.; Engelmann, R.; Farley, J.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Ahmad, A.; Arfaoui, S.; Devetak, E.; DeWilde, B.; Engelmann, R.; Farley, J.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Bartsch, V.; De Santo, A.; Martin-Haugh, S.; Potter, C. J.; Rose, A.; Salvatore, F.; Sutton, M. R.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Bangert, A.; Cuthbert, C.; Patel, N.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Waugh, A. T.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Chu, M. L.; Hou, S.; Lee, S. C.; Lin, S. C.; Liu, D.; Mazini, R.; Meng, Z.; Ren, Z. L.; Soh, D. A.; Teng, P. K.; Wang, J.; Wang, S. M.; Weng, Z.; Zhou, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Harpaz, S. Behar; Kajomovitz, E.; Rozen, Y.; Tarem, S.; Vallecorsa, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Bella, G.; Benary, O.; Benhammou, Y.; Canepa, A.; Dohmae, T.; Etzion, E.; Gershon, A.; Ginzburg, J.; Guttman, N.; Hod, N.; Munwes, Y.; Orem, Y.; Reinherz-Aronis, E.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Iliadis, D.; Kordas, K.; Kouskoura, V.; Nomidis, I.; Petridis, A.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, K.; Nakamura, T.; Ninomiyal, Y.; Okuyama, T.; Sakamoto, H.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yamazaki, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, K.; Nakamura, T.; Ninomiyal, Y.; Okuyama, T.; Sakamoto, H.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yamazaki, T.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Ishitsuka, M.; Jinnouchi, O.; Kanno, T.; Kuze, M.; Nobe, T.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Bailey, D. C.; Bain, T.; Brelier, B.; Cheung, S. L.; Dhaliwal, S.; Farooque, T.; Fatholahzadeh, B.; Gibson, A.; Guo, B.; Ilic, N.; Keung, J.; Knecht, N. S.; Krieger, P.; Le Maner, C.; Martensla, F. K.; Orr, R. S.; Rezvani, R.; Rosenbaum, G. A.; Savard, P.; Sinervo, P.; Spreitzer, T.; Tardif, D.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Chekulaev, S. V.; Fortin, D.; Koutsman, A.; Losty, M. J.; Nugent, I. M.; Oram, C. J.; Perez Codina, E.; Schouten, D.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hanawa, K.; Hara, K.; Hayashi, T.; Kim, S. H.; Kurata, M.; Nagai, K.; Ukegawa, F.] Univ Tsukuba, Inst Pure & Appl Sci, Tsukuba, Ibaraki 3058571, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Napier, A.; Rolli, S.; Sliwa, K.; Todorova-Nova, S.; Wetter, J.] Tufts Univ, Sci & Technol Ctr, Medford, MA USA. [Losada, M.; Loureiro, K. F.; Mendoza Navas, L.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Avolio, G.; Deng, J.; Farrell, S.; Eschrich, I. Gough; Hawkins, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Scannicchio, D. A.; Schernau, M.; Taffard, A.; Toggerson, B.; Unel, G.; Werth, M.; Wheeler-Ellis, S. J.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Del Papa, C.; Pinamonti, M.; Shaw, K.; Soualah, R.] Ist Nazl Fis Nucl, Grp Coll Udine, Udine, Italy. [Acharya, B. S.] ICTP, Udine, Italy. [Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Del Papa, C.; Giordani, M. P.; Pinamonti, M.; Shaw, K.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Benekos, N.; Coggeshall, J.; Cortes-Gonzalez, A.; Errede, D.; Errede, S.; Khandanyan, H.; Lie, K.; Liss, T. M.; McCarn, A.; Neubauer, M. S.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Brenner, R.; Buszello, C. P.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Pelikan, D.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.; Wildauer, A.] Univ Valencia, IFIC, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.; Wildauer, A.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.; Wildauer, A.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.; Wildauer, A.] Univ Valencia, IMB, CNM, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.; Wildauer, A.] CSIC, Valencia, Spain. [Axen, D.; Gay, C.; Gecse, Z.; Loh, C. W.; Mills, W. J.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Astbury, A.; Bansal, V.; Berghaus, F.; Courneyea, L.; Fincke-Keeler, M.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Lessard, J-R.; Marino, C. P.; Martyniuk, A. C.; McPherson, R. A.; Ouellette, E. A.; Plamondon, M.; Sobie, R.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Farrington, S. M.; Jones, G.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Kimura, N.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Alon, R.; Barak, L.; Bressler, S.; Duchovni, E.; Frank, T.; Gabizon, O.; Gross, E.; Groth-Jensen, J.; Klier, A.; Lellouch, D.; Levinson, L. 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[Amorim, A.; Gomes, A.; Maio, A.; Pina, J.] Univ Lisbon, CFNUL, Lisbon, Portugal. [Apolle, R.; Davies, E.; Mattravers, C.; Nash, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Azuelos, G.; Gingrich, D. M.; Oakham, F. G.; Savard, P.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Bawa, H. S.; Gao, Y. S.; Lowe, A. J.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beloborodova, O.; Talyshev, A.; Tikhonov, Y. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Canelli, F.] Fermilab Natl Accelerator Lab, Batavia, IL USA. [Carvalho, J.; Fiolhais, M. C. N.; Oliveira, M.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Castaneda Hernandez, A. M.] UASLP, Dept Phys, San Luis Potosi, Mexico. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Demirkoz, B.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Dhullipudi, R.; Greenwood, Z. D.; Sawyer, L.] Louisiana Tech Univ, Ruston, LA 71270 USA. 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Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Olshevskiy, Alexander/I-1580-2016; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Grancagnolo, Sergio/J-3957-2015; spagnolo, stefania/A-6359-2012; Shmeleva, Alevtina/M-6199-2015; Camarri, Paolo/M-7979-2015; Gavrilenko, Igor/M-8260-2015; Tikhomirov, Vladimir/M-6194-2015; Chekulaev, Sergey/O-1145-2015; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; Carvalho, Joao/M-4060-2013; Mashinistov, Ruslan/M-8356-2015; Booth, Christopher/B-5263-2016; Ventura, Andrea/A-9544-2015; Livan, Michele/D-7531-2012; Mitsou, Vasiliki/D-1967-2009; Joergensen, Morten/E-6847-2015; Mir, Lluisa-Maria/G-7212-2015; Riu, Imma/L-7385-2014; Garcia, Jose /H-6339-2015; Della Pietra, Massimo/J-5008-2012; Cavalli-Sforza, Matteo/H-7102-2015; Petrucci, Fabrizio/G-8348-2012; Negrini, Matteo/C-8906-2014; Ferrer, Antonio/H-2942-2015; Hansen, John/B-9058-2015; Kupco, Alexander/G-9713-2014; Mikestikova, Marcela/H-1996-2014; Kuday, Sinan/C-8528-2014; Snesarev, Andrey/H-5090-2013; Svatos, Michal/G-8437-2014; Chudoba, Jiri/G-7737-2014; Peleganchuk, Sergey/J-6722-2014; Santamarina Rios, Cibran/K-4686-2014; Bosman, Martine/J-9917-2014; Lei, Xiaowen/O-4348-2014; Demirkoz, Bilge/C-8179-2014; Gutierrez, Phillip/C-1161-2011; De, Kaushik/N-1953-2013; Sukharev, Andrey/A-6470-2014; Fazio, Salvatore /G-5156-2010; Lee, Jason/B-9701-2014; Robson, Aidan/G-1087-2011; Smirnova, Oxana/A-4401-2013; Fabbri, Laura/H-3442-2012; Villa, Mauro/C-9883-2009; Kepka, Oldrich/G-6375-2014; Nemecek, Stanislav/G-5931-2014; Jakoubek, Tomas/G-8644-2014; Lokajicek, Milos/G-7800-2014; Staroba, Pavel/G-8850-2014; Kuleshov, Sergey/D-9940-2013; Anjos, Nuno/I-3918-2013; Kartvelishvili, Vakhtang/K-2312-2013; Prokoshin, Fedor/E-2795-2012; Dawson, Ian/K-6090-2013; Ferrando, James/A-9192-2012; Tudorache, Valentina/D-2743-2012; Marti-Garcia, Salvador/F-3085-2011; Castro, Nuno/D-5260-2011; Wolters, Helmut/M-4154-2013; Brooks, William/C-8636-2013; Warburton, Andreas/N-8028-2013 OI Vanyashin, Aleksandr/0000-0002-0367-5666; Moorhead, Gareth/0000-0002-9299-9549; Stoicea, Gabriel/0000-0002-7511-4614; Doyle, Anthony/0000-0001-6322-6195; Pina, Joao /0000-0001-8959-5044; Solfaroli Camillocci, Elena/0000-0002-5347-7764; La Rosa, Alessandro/0000-0001-6291-2142; Smirnov, Sergei/0000-0002-6778-073X; Conde Muino, Patricia/0000-0002-9187-7478; Andreazza, Attilio/0000-0001-5161-5759; Boyko, Igor/0000-0002-3355-4662; Veloso, Filipe/0000-0002-5956-4244; Gomes, Agostinho/0000-0002-5940-9893; la rotonda, laura/0000-0002-6780-5829; Osculati, Bianca Maria/0000-0002-7246-060X; Amorim, Antonio/0000-0003-0638-2321; Coccaro, Andrea/0000-0003-2368-4559; Korol, Aleksandr/0000-0001-8448-218X; Maio, Amelia/0000-0001-9099-0009; Fiolhais, Miguel/0000-0001-9035-0335; Karyukhin, Andrey/0000-0001-9087-4315; Anjos, Nuno/0000-0002-0018-0633; Giordani, Mario/0000-0002-0792-6039; Abdelalim, Ahmed Ali/0000-0002-2056-7894; Capua, Marcella/0000-0002-2443-6525; Di Micco, Biagio/0000-0002-4067-1592; Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; Doria, Alessandra/0000-0002-5381-2649; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Maneira, Jose/0000-0002-3222-2738; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Goncalo, Ricardo/0000-0002-3826-3442; Gauzzi, Paolo/0000-0003-4841-5822; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Monzani, Simone/0000-0002-0479-2207; Grancagnolo, Francesco/0000-0002-9367-3380; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Wemans, Andre/0000-0002-9669-9500; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Olshevskiy, Alexander/0000-0002-8902-1793; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Grancagnolo, Sergio/0000-0001-8490-8304; spagnolo, stefania/0000-0001-7482-6348; Camarri, Paolo/0000-0002-5732-5645; Tikhomirov, Vladimir/0000-0002-9634-0581; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; Carvalho, Joao/0000-0002-3015-7821; Mashinistov, Ruslan/0000-0001-7925-4676; Booth, Christopher/0000-0002-6051-2847; Ventura, Andrea/0000-0002-3368-3413; Livan, Michele/0000-0002-5877-0062; Mitsou, Vasiliki/0000-0002-1533-8886; Joergensen, Morten/0000-0002-6790-9361; Mir, Lluisa-Maria/0000-0002-4276-715X; Riu, Imma/0000-0002-3742-4582; Della Pietra, Massimo/0000-0003-4446-3368; Petrucci, Fabrizio/0000-0002-5278-2206; Negrini, Matteo/0000-0003-0101-6963; Ferrer, Antonio/0000-0003-0532-711X; Hansen, John/0000-0002-8422-5543; Mikestikova, Marcela/0000-0003-1277-2596; Kuday, Sinan/0000-0002-0116-5494; Svatos, Michal/0000-0002-7199-3383; Peleganchuk, Sergey/0000-0003-0907-7592; Santamarina Rios, Cibran/0000-0002-9810-1816; Bosman, Martine/0000-0002-7290-643X; Lei, Xiaowen/0000-0002-2564-8351; De, Kaushik/0000-0002-5647-4489; Lee, Jason/0000-0002-2153-1519; Smirnova, Oxana/0000-0003-2517-531X; Fabbri, Laura/0000-0002-4002-8353; Villa, Mauro/0000-0002-9181-8048; Kuleshov, Sergey/0000-0002-3065-326X; Prokoshin, Fedor/0000-0001-6389-5399; Ferrando, James/0000-0002-1007-7816; Castro, Nuno/0000-0001-8491-4376; Wolters, Helmut/0000-0002-9588-1773; Brooks, William/0000-0001-6161-3570; Warburton, Andreas/0000-0002-2298-7315 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union; ERC, European Union; NSRF, European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; ISF, Israel; MINERVA, Israel; GIF, Israel; DIP, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; GRICES, Portugal; FCT, Portugal; MERYS (MECTS), Romania; MES of Russia; ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MVZT, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America; SER, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; ISF, MINERVA, GIF, DIP and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW, Poland; GRICES and FCT, Portugal; MERYS (MECTS), Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MVZT, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. NR 69 TC 24 Z9 24 U1 9 U2 136 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD JAN PY 2013 VL 73 IS 1 AR 2261 DI 10.1140/epjc/s10052-012-2261-1 PG 28 WC Physics, Particles & Fields SC Physics GA 135KX UT WOS:000318288100002 ER PT J AU Aad, G Abajyan, T Abbott, B Abdallah, J Khalek, SA Abdelalim, AA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Acharya, BS Adamczyk, L Adams, DL Addy, TN Adelman, J Adomeit, S Adragna, P Adye, T Aefsky, S Aguilar-Saavedra, JA Agustoni, M Aharrouche, M Ahlen, SP Ahles, F Ahmad, A Ahsan, M Aielli, G Akdogan, T Akesson, TPA Akimoto, G Akimov, AV Alam, MS Alam, MA Albert, J Albrand, S Aleksa, M Aleksandrov, IN Alessandria, F Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Aliev, M Alimonti, G Alison, J Allbrooke, BMM Allport, PP Allwood-Spiers, SE Almond, J Aloisio, A Alon, R Alonso, A Alonso, F Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Amelung, C Ammosov, VV Dos Santos, SPA Amorim, A Amram, N Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Andrieux, ML Anduaga, XS Angelidakis, S Anger, P Angerami, A Anghinolfi, F Anisenkov, A Anjos, N Annovi, A Antonaki, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Aoun, S Bella, LA Apolle, R Arabidze, G Aracena, I Arai, Y Arce, ATH Arfaoui, S Arguin, JF Arik, E Arik, M Armbruster, AJ Arnaez, O Arnal, V Arnault, C Artamonov, A Artoni, G Arutinov, D Asai, S Ask, S Asman, B Asquith, L Assamagan, K Astbury, A Atkinson, M Aubert, B Auge, E Augsten, K Aurousseau, M Avolio, G Avramidou, R Axen, D Azuelos, G Azuma, Y Baak, MA Baccaglioni, G Bacci, C Bach, AM Bachacou, H Bachas, K Backes, M Backhaus, M Mayes, JB Badescu, E Bagnaia, P Bahinipati, S Bai, Y Bailey, DC Bain, T Baines, JT Baker, OK Baker, MD Baker, S Balek, P Banas, E Banerjee, P Banerjee, S Banfi, D Bangert, A Bansal, V Bansil, HS Barak, L Baranov, SP Galtieri, AB Barber, T Barberio, EL Barberis, D Barbero, M Bardin, DY Barillari, T Barisonzi, M Barklow, T Barlow, N Barnett, BM Barnett, RM Baroncelli, A Barone, G Barr, AJ Barreiro, F Da Costa, JBG Barrillon, P Bartoldus, R Barton, AE Bartsch, V Basye, A Bates, RL Batkova, L Batley, JR Battaglia, A Battistin, M Bauer, F Bawa, HS Beale, S Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, AK Becker, S Beckingham, M Becks, KH Beddall, AJ Beddall, A Bedikian, S Bednyakov, VA Bee, CP Beemster, LJ Begel, M Harpaz, SB Behera, PK Beimforde, M Belanger-Champagne, C Bell, PJ Bell, WH Bella, G Bellagamba, L Bellomo, M Belloni, A Beloborodova, O Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Benoit, M Bensinger, JR Benslama, K Bentvelsen, S Berge, D Kuutmann, EB Berger, N Berghaus, F Berglund, E Beringer, J Bernat, P Bernhard, R Bernius, C Berry, T Bertella, C Bertin, A Bertolucci, F Besana, MI Besjes, GJ Besson, N Bethke, S Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Bieniek, SP Bierwagen, K Biesiada, J Biglietti, M Bilokon, H Bindi, M Binet, S Bingul, A 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Zobernig, G. Zoccoli, A. Nedden, M. Zur Zutshi, V. Zwalinski, L. CA ATLAS Collaboration TI Search for pair-produced massive coloured scalars in four-jet final states with the ATLAS detector in proton-proton collisions at root s=7 TeV SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID SUPERSYMMETRY AB A search for pair-produced massive coloured scalar particles decaying to a four-jet final state is performed by the ATLAS experiment at the LHC in proton-proton collisions at root s = 7 TeV. The analysed data sample corresponds to an integrated luminosity of 4.6 fb(-1). No deviation from the Standard Model is observed in the invariant mass spectrum of the two-jet pairs. A limit on the scalar gluon pair production cross section of 70 pb (10 pb) is obtained at the 95 % confidence level for a scalar gluon mass of 150 GeV (350 GeV). Interpreting these results as mass limits on scalar gluons, masses ranging from 150 GeV to 287 GeV are excluded at the 95 % confidence level. 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D.; Ruckstuhl, N.; Tsipolitis, G.; Vlachos, S.] Natl Tech Univ Athens, Dept Phys, Zografos, Greece. [Abdinov, O.; Khalilzada, F.] Azerbaijan Acad Sci, Inst Phys, Baku 370143, Azerbaijan. [Abdallah, J.; Bosman, M.; Armadans, R. Caminal; Casado, M. P.; Cavalli-Sforza, M.; Conidi, M. C.; Demirkoz, B.; Curull, X. Espinal; Francavilla, P.; Giangiobbe, V.; Parra, G. Gonzalez; Grinstein, S.; Helsens, C.; Rozas, A. Juste; Korolkov, I.; Le Menedeu, E.; Martinez, M.; Mir, L. M.; Berlingen, J. Montejo; Nadal, J.; Osuna, C.; Pages, A. Pacheco; Aranda, C. Padilla; Riu, I.; Rossetti, V.; Rubbo, F.; Succurro, A.; Tsiskaridze, S.; Vorwerk, V.] Univ Autonoma Barcelona, Inst Fis Altes Energies, E-08193 Barcelona, Spain. [Abdallah, J.; Bosman, M.; Armadans, R. Caminal; Casado, M. P.; Cavalli-Sforza, M.; Conidi, M. C.; Demirkoz, B.; Curull, X. Espinal; Francavilla, P.; Giangiobbe, V.; Parra, G. Gonzalez; Grinstein, S.; Helsens, C.; Rozas, A. Juste; Korolkov, I.; Le Menedeu, E.; Martinez, M.; Mir, L. M.; Berlingen, J. Montejo; Nadal, J.; Osuna, C.; Pages, A. Pacheco; Aranda, C. Padilla; Riu, I.; Rossetti, V.; Rubbo, F.; Succurro, A.; Tsiskaridze, S.; Vorwerk, V.] Univ Autonoma Barcelona, Dept Fis, E-08193 Barcelona, Spain. [Abdallah, J.; Bosman, M.; Armadans, R. Caminal; Casado, M. P.; Cavalli-Sforza, M.; Conidi, M. C.; Demirkoz, B.; Curull, X. Espinal; Francavilla, P.; Giangiobbe, V.; Parra, G. Gonzalez; Grinstein, S.; Helsens, C.; Rozas, A. Juste; Korolkov, I.; Le Menedeu, E.; Martinez, M.; Mir, L. M.; Berlingen, J. Montejo; Nadal, J.; Osuna, C.; Pages, A. Pacheco; Aranda, C. Padilla; Riu, I.; Rossetti, V.; Rubbo, F.; Succurro, A.; Tsiskaridze, S.; Vorwerk, V.] ICREA, Barcelona, Spain. [Borjanovic, I.; Krstic, J.; Popovic, D. S.; Sijacki, Dj.; Simic, Lj.] Univ Belgrade, Inst Phys, Belgrade, Serbia. [Borjanovic, I.; Krstic, J.; Popovic, D. S.; Sijacki, Dj.; Simic, Lj.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia. [Buanes, T.; Burgess, T.; Eigen, G.; Kastanas, A.; Liebig, W.; Lipniacka, A.; Rosendahl, P. L.; Sandaker, H.; Sjursen, T. B.; Stugu, B.; Tonoyan, A.; Ugland, M.] Univ Bergen, Dept Phys & Techol, Bergen, Norway. [Bach, A. M.; Galtieri, A. Barbaro; Barnett, R. M.; Beringer, J.; Biesiada, J.; Calafiura, P.; Caminada, L. M.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Copic, K.; Dube, S.; Einsweiler, K.; Gaponenko, A.; Garcia-Sciveres, M.; Gilehriese, M.; Haber, C.; Hance, M.; Heinemann, B.; Hinchliffe, I.; Hsu, S. -C.; Hurwitz, M.; Lavrijsen, W.; Loscutoff, P.; Madaras, R. J.; Ovcharova, A.; Griso, S. Pagan; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Skinnari, L. A.; Tatarkhanov, M.; Tibbetts, M. J.; Tsulaia, V.; Vahsen, S.; Varouchas, D.; Virzi, J.; Yao, Y.; Zenz, S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Phys, Berkeley, CA 94720 USA. [Bach, A. M.; Galtieri, A. Barbaro; Barnett, R. M.; Beringer, J.; Biesiada, J.; Calafiura, P.; Caminada, L. M.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Copic, K.; Dube, S.; Einsweiler, K.; Gaponenko, A.; Garcia-Sciveres, M.; Gilehriese, M.; Haber, C.; Hance, M.; Heinemann, B.; Hinchliffe, I.; Hsu, S. -C.; Hurwitz, M.; Lavrijsen, W.; Loscutoff, P.; Madaras, R. J.; Ovcharova, A.; Griso, S. Pagan; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Skinnari, L. A.; Tatarkhanov, M.; Tibbetts, M. J.; Tsulaia, V.; Vahsen, S.; Varouchas, D.; Virzi, J.; Yao, Y.; Zenz, S.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Aliev, M.; Giorgi, F. M.; Grancagnolo, S.; Herrberg, R.; Hristova, I.; Kind, O.; Kolanoski, H.; Kwee, R.; Lacker, H.; Leyton, M.; Lohse, T.; Mandrysch, R.; Nikiforov, A.; Schulz, H.; Wendland, D.; Nedden, M. Zur] Humboldt Univ, Dept Phys, Berlin, Germany. [Agustoni, M.; Ancu, L. S.; Battaglia, A.; Beck, H. P.; Borer, C.; Ereditato, A.; Martin, T. Fonseca; Gallo, V.; Haug, S.; Kabana, S.; Kruker, T.; Marti, L. F.; Pretzl, K.; Schneider, B.; Topfel, C.; Weber, M. S.] Univ Bern, Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Agustoni, M.; Ancu, L. S.; Battaglia, A.; Beck, H. P.; Borer, C.; Ereditato, A.; Martin, T. Fonseca; Gallo, V.; Haug, S.; Kabana, S.; Kruker, T.; Marti, L. F.; Pretzl, K.; Schneider, B.; Topfel, C.; Weber, M. S.] Univ Bern, High Energy Phys Lab, Bern, Switzerland. [Allbrooke, B. M. M.; Bansil, H. S.; Bracinik, J.; Charlton, D. G.; Chisholm, A. S.; Collins, N. J.; Curtis, C. J.; Hadley, D. R.; Hawkes, C. M.; Head, S. J. 018; Hillier, S. J.; Mahout, G.; Martin, T. A.; Mclaughlan, T.; Newman, P. R.; Nikolopoulos, K.; Palmer, J. D.; Slater, M.; Thomas, J. P.; Thompson, P. D.; Watkins, P. M.; Watson, A. T.; Watson, M. F.; Wilson, J. A.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Akdogan, T.; Arik, E.; Arik, M.; Istin, S.; Ozcan, V. E.; Rador, T.] Bogazici Univ, Dept Phys, Istanbul, Turkey. [Cetin, S. A.] Dogus Univ, Div Phys, Istanbul, Turkey. [Beddall, A. J.; Beddall, A.; Bingul, A.] Gaziantep Univ, Dept Engn Phys, Gaziantep, Turkey. Istanbul Tech Univ, Dept Phys, TR-80626 Istanbul, Turkey. [Bellagamba, L.; Bertin, A.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; Caforio, D.; Ciocca, C.; Corradi, M.; De Castro, S.; Di Sipio, R.; Fabbri, L.; Giacobbe, B.; Giusti, P.; Grafstrom, P.; Jha, M. K.; Massa, I.; Mengarelli, A.; Monzani, S.; Negrini, M.; Piccinini, M.; Polini, A.; Rinaldi, L.; Romano, M.; Sbarra, C.; Semprini-Cesari, N.; Spighi, R.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Bertin, A.; Caforio, D.; Ciocca, C.; De Castro, S.; Di Sipio, R.; Fabbri, L.; Grafstrom, P.; Massa, I.; Mengarelli, A.; Monzani, S.; Piccinini, M.; Romano, M.; Semprini-Cesari, N.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, Dipartmento Fis, Bologna, Italy. [Abajyan, T.; Arutinov, D.; Backhaus, M.; Barbero, M.; Bechtle, P.; Brock, I.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Gaycken, G.; Geich-Gimbel, Ch.; Glatzer, J.; Gonella, L.; Haefner, P.; Havranek, M.; Hellmich, D.; Hillert, S.; Huegging, E.; Karagounis, M.; Khoriauli, G.; Koevesarki, P.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lapoire, C.; Lehmacher, M.; Leyko, A. M.; Limbach, C.; Loddenkoetter, T.; Mazur, M.; Moser, N.; Mueller, K.; Nattermann, T.; Nuncio-Quiroz, A. -E.; Pohl, D.; Psoroulas, S.; Schaepe, S.; Schmieden, K.; Schmitz, M.; Schultens, M. J.; Schwindt, T.; Stillings, J. A.; Therhaag, J.; Tsung, J. -W.; Uchida, K.; Uhlenbrock, M.; Urquijo, P.; Vogel, A.; Von Toerne, E.; Wang, T.; Wermes, N.; Wienemann, P.; Wiikfuchs, L. A. M.; Zendler, C.; Zimmermann, R.; Zimmermann, S.] Univ Bonn, Inst Phys, Bonn, Germany. [Ahlen, S. P.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, Boston, MA 02215 USA. [Aefsky, S.; Amelung, C.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Daya-Ishmukhametova, R. K.; Gozpinar, S.; Pomeroy, D.; Sciolla, G.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Caloba, L. P.; Maidantchik, C.; Marroquim, E.; Nepomuceno, A. A.; Perantoni, M.; Seixas, J. M.] Univ Fed Rio De Janeiro COPPE EE IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; Manhaes de Andrade Filho, L.] Fed Univ Juiz de Fora UFJF, Juiz De Fora, Brazil. [do Vale, M. A. B.] Fed Univ Sao Joao Del Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadelli, M.; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Baker, M. D.; Begel, M.; Bernius, C.; Chen, H.; Chernyatin, V.; Debbe, R.; Dhullipudi, R.; Ernst, M.; Gadfort, T.; Gibbard, B.; Gordon, H. A.; Greenwood, Z. D.; Klimentov, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Majewski, S.; Metcalfe, J.; Nevski, P.; Okawa, H.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Park, W.; Pleier, M. -A.; Poblaguev, A.; Polychronakos, V.; Pravahan, R.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rahm, D.; Rajagopalan, S.; Redlinger, G.; Sawyer, L.; Sircar, A.; Snyder, S.; Steinberg, P.; Stumer, I.; Subramaniam, R.; Takai, H.; Tamsett, M. C.; Triplett, N.; Undrus, A.; Wenaus, T.; Ye, S.; Yu, D.; Zaytsev, A.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Badescu, E.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Cuciuc, C. -M.; Dinut, F.; Dita, P.; Dita, S.; Micu, L.; Olari, A.; Pantea, D.; Popeneciu, G. A.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Darlea, G. L.] Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Silva, M. L. Gonzalez; Garzon, G. Otero Y.; Piegaia, R.; Romeo, G.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Ask, S.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Buttinger, W.; Carter, J. R.; Chapman, J. D.; Cowden, C.; French, S. T.; Frost, J. A.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Moeller, V.; Parker, M. A.; Robinson, D.; Sandoval, T.; Thomson, M.; Ward, C. P.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Gillberg, D.; Koffas, T.; Lacey, J.; Liu, C.; Marchand, J. F.; McCarthy, T. G.; Oakham, F. G.; Randrianarivony, K.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Anastopoulos, C.; Avolio, G.; Baak, M. A.; Bachas, K.; Banfi, D.; Battistin, M.; Bellomo, M.; Beltramello, O.; Berge, D.; Bianchi, R. M.; Blanchot, G.; Bogaerts, J. A.; Boyd, J.; Bremer, J.; Burckhart, H.; Byszewski, M.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Catmore, J. 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Lehmann; Lenzi, B.; Lichard, P.; Malaescu, B.; Malyukov, S.; Mapelli, A.; Mapelli, L.; Marshall, Z.; Martin, B.; Messina, A.; Meyer, T. C.; Michal, S.; Molfetas, A.; Morley, A. K.; Mornacchi, G.; Muenstermann, D.; Nairz, A. M.; Nakahama, Y.; Negri, G.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Ohm, C. C.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Petersen, J.; Piacquadio, G.; Pommes, K.; Poppleton, A.; Bueso, X. Portell; Poulard, G.; Prasad, S.; Raymond, M.; Rembser, C.; Dos Santos, D. Roda; Roe, S.; Salek, D.; Salzburger, A.; Savu, D. O.; Schlenker, S.; Schott, M.; Sfyrla, A.; Spigo, G.; Spiwoks, R.; Stewart, G. A.; Teischinger, F. A.; Ten Kate, H.; Torchiani, I.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; Van der Ster, D.; Van Eldik, N.; Vandelli, W.; Veness, R.; Vinek, E.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. 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[Han, L.; Jiang, Y.; Li, S.; Liu, M.; Liu, Y.; Peng, H.; Wang, H.; Wu, Y.; Xu, C.; Zhang, D.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Feng, C.; Ge, P.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Toro, R. Camacho; Cinca, D.; Donini, J.; Febbraro, R.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Vazeille, F.] Clermont Univ, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Toro, R. Camacho; Cinca, D.; Donini, J.; Febbraro, R.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Toro, R. Camacho; Cinca, D.; Donini, J.; Febbraro, R.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Vazeille, F.] Univ Clermont Ferrand, Photochim Mol & Macromol Lab, CNRS, IN2P3, F-63177 Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Brooijmans, G.; Chen, Y.; Dodd, J.; Grau, N.; Guo, J.; Hu, D.; Hughes, E. W.; Nikiforou, N.; Parsons, J. A.; Penson, A.; Perez, K.; Reale, V. Perez; Scherzer, M. I.; Spousta, M.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Williams, E.; Willis, W.; Wulf, E.; Zivkovic, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Boelaert, N.; Dam, M.; Gregersen, K.; Hansen, J. R.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Heisterkamp, S.; Jakobsen, S.; Loevschall-Jensen, A. E.; Jez, P.; Joergensen, M. D.; Kadlecik, P.; Klinkby, E. B.; Lundquist, J.; Mackeprang, R.; Mehlhase, S.; Petersen, T. C.; Simonyan, M.; Thomsen, L. A.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; Fazio, S.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Morello, G.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Grp Collegato Cosenza, Arcavacata Di Rende, Italy. [Capua, M.; Crosetti, G.; Fazio, S.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Morello, G.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Banas, E.; Blocki, J.; De Renstrom, P. A. Bruckman; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Malecki, P.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Turala, M.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.; Zemla, A.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Yagci, K. Dindar; Firan, A.; Hoffman, J.; Joffe, D.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Rios, R. R.; Sekula, S. J.; Stroynowski, R.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Ahsan, M.; Izen, J. M.; Lou, X.; Reeves, K.; Wong, W. C.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Kuutmann, E. Bergeaas; Bloch, I.; Dassoulas, J. A.; Dietrich, J.; Ehrenfeld, W.; Ferrara, V.; Fischer, G.; Friedrich, C.; Glazov, A.; Goebel, M.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Gosdzik, B.; Grahn, K-J.; Gregor, I. M.; Hiller, K. H.; Huettmann, A.; Belenguer, M. Jimenez; Johnert, S.; Karnevskiy, M.; Katzy, J.; Kono, T.; Kuhl, T.; Lange, C.; Lobodzinska, E.; Ludwig, D.; Medinnis, M.; Monig, K.; Naumann, T.; Cavalcanti, T. Perez; Petschull, D.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Zhu, H.] DESY, Hamburg, Germany. [Kuutmann, E. Bergeaas; Bloch, I.; Dassoulas, J. A.; Dietrich, J.; Ehrenfeld, W.; Ferrara, V.; Fischer, G.; Friedrich, C.; Glazov, A.; Goebel, M.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Gosdzik, B.; Grahn, K-J.; Gregor, I. M.; Hiller, K. H.; Huettmann, A.; Belenguer, M. Jimenez; Johnert, S.; Karnevskiy, M.; Katzy, J.; Kono, T.; Kuhl, T.; Lange, C.; Lobodzinska, E.; Ludwig, D.; Medinnis, M.; Monig, K.; Naumann, T.; Cavalcanti, T. Perez; Petschull, D.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. 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[Annovi, A.; Antonelli, M.; Bilokon, H.; Cerutti, F.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.; Volpi, G.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Aad, G.; Ahles, F.; Barber, T.; Bernhard, R.; Boehler, M.; Bruneliere, R.; Christov, A.; Consorti, V.; Fehling-Kaschek, M.; Flechl, M.; Hartert, J.; Herten, G.; Horner, S.; Jakobs, K.; Janus, M.; Kononov, A. I.; Kuehn, S.; Lai, S.; Landgraf, U.; Lohwasser, K.; Ludwig, I.; Ludwig, J.; Mahboubi, K.; Mohr, W.; Nilsen, H.; Parzefall, U.; Rammensee, M.; Rave, T. C.; Rurikova, Z.; Schmidt, E.; Schumacher, M.; Siegert, F.; Stoerig, K.; Sundermann, J. E.; Temming, K. K.; Thoma, S.; Tsiskaridze, V.; Venturi, M.; Vivarelli, I.; Von Radziewski, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Winkelmann, S.; Xie, S.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Abdelalim, A. A.; Alexandre, G.; Backes, M.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; Blondel, A.; Bucci, F.; Clark, A.; Dao, V.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Iacobucci, G.; La Rosa, A.; Lister, A.; Latour, B. Martin Dit; Mermod, P.; Herrera, C. Mora; Nektarijevic, S.; Nessi, M.; Nikolics, K.; Pasztor, G.; Picazio, A.; Pohl, M.; Rosbach, K.; Rosselet, L.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Beccherle, R.; Caso, C.; Dameri, M.; Darbo, G.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Barberis, D.; Caso, C.; Dameri, M.; Parodi, A. Ferretto; Gagliardi, G.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Chikovani, L.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Khubua, J.; Mchedlidze, G.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Stenzel, H.] Univ Giessen, Inst Phys 2, D-35390 Giessen, Germany. [Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Bussey, P.; Buttar, C. M.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Edwards, N. C.; Ferrag, S.; Ferrando, J.; De Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Kar, D.; Kenyon, M.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Robson, A.; Saxon, D. H.; Smith, K. M.; Denis, R. D. St.; Steele, G.; Thompson, A. S.; Wraight, K.; Wright, M.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bierwagen, K.; Blumenschein, U.; Brandt, O.; Erdmann, J.; Evangelakou, D.; George, M.; Grosse-Knetter, J.; Guindon, S.; Hamer, M.; Hensel, C.; Keil, M.; Knue, A.; Kohn, F.; Krieger, N.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Mann, A.; Meyer, J.; Morel, J.; Nackenhorst, O.; Pashapour, S.; Quadt, A.; Roe, A.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Uhrmacher, M.; Schroeder, T. Vazquez; Weber, P.; Weingarten, J.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Andrieux, M-L.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Stark, J.; Sun, X.; Trocme, B.; Wang, J.; Weydert, C.] Univ Grenoble 1, Lab Phys Subatom & Cosmol, Grenoble, France. [Albrand, S.; Andrieux, M-L.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Stark, J.; Sun, X.; Trocme, B.; Wang, J.; Weydert, C.] CNRS, IN2P3, Grenoble, France. [Albrand, S.; Andrieux, M-L.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Stark, J.; Sun, X.; Trocme, B.; Wang, J.; Weydert, C.] Inst Natl Polytech Grenoble, F-38031 Grenoble, France. [Addy, T. N.; Harvey, A.; McFarlane, K. W.; Shin, T.; Vassilakopoulos, V. I.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Da Costa, J. Barreiro Guimaraes; Belloni, A.; Catastini, P.; Conti, G.; Franklin, M.; Huth, J.; Jeanty, L.; Kagan, M.; Mateos, D. Lopez; Outschoorn, V. Martinez; Mercurio, K. M.; Mills, C.; Morii, M.; Skottowe, H. P.; Smith, B. C.; Della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Anders, G.; Andrei, V.; Davygora, Y.; Dietzsch, T. A.; Dunford, M.; Geweniger, C.; Hanke, P.; Henke, M.; Khomich, A.; Kluge, E. -E.; Lang, V. S.; Lendermann, V.; Lepolda, F.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Kugel, A.; Maenner, R.; Schroer, N.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Cwetanski, P.; Evans, H.; Gagnon, P.; Jain, V.; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Price, D.; Whittington, D.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Epp, B.; Jussel, P.; Kneringer, E.; Kuhn, D.; Lukas, W.; Rudolph, G.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Behera, P. K.; Limper, M.; Mallik, U.; Pylypchenko, Y.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Rosenberg, E. I.; Ruiz-Martinez, A.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Aleksandrov, I. N.; Bardin, D. Y.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Grigalashvili, N.; Huseynov, N.; Kalinovskaya, L. V.; Kazarinov, M. Y.; Kekelidze, G. D.; Kharchenko, D.; Khramov, E.; Kolesnikov, V.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Pozdnyakov, V.; Rumyantsev, L.; Rusakovich, N. A.; Sadykov, R.; Shiyakova, M.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.; Zimin, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Arai, Y.; Doi, Y.; Haruyama, T.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Makida, Y.; Manabe, A.; Mitsui, S.; Nagano, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Hayakawa, T.; King, M.; Kishimoto, T.; Kitamura, T.; Kurashige, H.; Matsushita, T.; Ochi, A.; Suzuki, Y.; Takeda, H.; Tani, K.; Watanabe, I.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Sasao, N.; Sumida, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Davidson, R.; De Mora, L.; Dearnaley, W. J.; Fox, H.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Bianco, M.; Cataldi, G.; Chiodini, G.; Gorini, E.; Grancagnolo, F.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Bianco, M.; Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Greenshaw, T.; Gwilliam, C. B.; Hayward, H. S.; Jackson, J. N.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kluge, T.; Kretzschmar, J.; Laycock, P.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Sellers, G.; Vossebeld, J. H.; Waller, P.; Wrona, B.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Dolenc, I.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Dolenc, I.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia. [Adragna, P.; Bona, M.; Carter, A. A.; Cerrito, L.; Eisenhandler, E.; Ellis, K.; Goddard, J. R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Poll, J.; Rizvi, E.; Salamanna, G.; Castanheira, M. Teixeira Dias; Wiglesworth, C.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Alam, M. A.; Berry, T.; Boisvert, V.; Brooks, T.; Cantrill, R.; Cowan, G.; Duguid, L.; Edwards, C. A.; George, S.; Goncalo, R.; Hayden, D.; Vazquez, J. G. Panduro; Pastore, Fr.; Rose, M.; Spano, F.; Strong, J. A.; Teixeira-Dias, P.] Royal Holloway Univ London, Dept Phys, London, Surrey, England. [Baker, S.; Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Chislett, R. T.; Christidi, I. A.; Cooper, B. D.; Davison, A. R.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Lambourne, L.; Monk, J.; Nash, M.; Nurse, E.; Prabhu, R.; Sherwood, P.; Simmons, B.; Taylor, C.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Cavalleri, P.; Chareyre, E.; Davignon, O.; De Cecco, S.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph.; Theveneaux-Pelzer, T.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Cavalleri, P.; Chareyre, E.; Davignon, O.; De Cecco, S.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph.; Theveneaux-Pelzer, T.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Cavalleri, P.; Chareyre, E.; Davignon, O.; De Cecco, S.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph.; Theveneaux-Pelzer, T.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Alonso, A.; Bocchetta, S. S.; Floderus, A.; Hawkins, A. D.; Hedberg, V. 079; Jarlskog, G.; Lundberg, B.; Lytken, E.; Meirose, B.; Mjornmark, J. U.; Smirnova, O.] Lund Univ, Fys Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Labarga, L.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Aharrouche, M.; Arnaez, O.; Blum, W.; Buescher, V.; Caputo, R.; Eckweiler, S.; Edmonds, K.; Ellinghaus, F.; Ertel, E.; Fiedler, F.; Fleckner, J.; Goeringer, C.; Handel, C.; Hohlfeld, M.; Hsu, P. J.; Ji, W.; Kawamura, G.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lungwitz, M.; Mattig, S.; Masetti, L.; Meyer, C.; Moreno, D.; Mueller, T.; Neusiedl, A.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schroeder, C.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Almond, J.; Borri, M.; Brown, G.; Chavda, V.; Cox, B. E.; Da Via, C.; Duerdoth, I. P.; Forti, A.; Howarth, J.; Ibbotson, M.; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Marx, M.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Pilkington, A. D.; Robinson, J. E. M.; Schwanenberger, C.; Snow, S. W.; Watts, S.; Woudstra, M. J.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aoun, S.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Moonier, E.; Odier, J.; Pralavorio, P.; Rozanov, A.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aoun, S.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Moonier, E.; Odier, J.; Pralavorio, P.; Rozanov, A.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Brau, B.; Colon, G.; Dallapiccola, C.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Caron, B.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Dobbs, M.; Dufour, M-A.; Klemetti, M.; Mc Donald, J.; Robertson, S. H.; Rios, C. Santamarina; Schram, M.; Stockton, M. C.; Vachon, B.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Davidson, N.; Diglio, S.; Hamano, K.; Jennens, D.; Kubota, T.; Limosani, A.; Moorhead, G. F.; Hanninger, G. Nunes; Phan, A.; Shao, Q. T.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Volpis, M.; White, M. J.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Armbruster, A. J.; Borroni, S.; Bortfeldt, J.; Chapman, J. W.; Cirilli, M.; Dai, T.; Diehl, E. B.; Ferretti, C.; Goldfarb, S.; Harper, D.; Levin, D.; Li, X.; Liu, H.; Liu, J. B.; Liu, L.; Mc Kee, S. P.; Neal, H. A.; Panikashvili, N.; Purdham, J.; Qian, J.; Scheirich, D.; Thun, R. P.; Walch, S.; Wilson, A.; Wooden, G.; Wu, Y.; Yang, H.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Fedorko, W.; Hauser, R.; Holzbauer, J. L.; Huston, J.; Koll, J.; Linnemann, J. T.; Mangeard, P. S.; Martin, B.; Miller, R. J.; Pope, B. G.; Schwienhorst, R.; Stelzer, H. J.; Tollefson, K.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alessandria, F.; Alimonti, G.; Andreazza, A.; Baccaglioni, G.; Besana, M. I.; Broggi, F.; Carminati, L.; Cavalli, D.; Citterio, M.; Consonni, S. M.; Costa, G.; Fanti, M.; Favareto, A.; Giugni, D.; Koletsou, I.; Laria, T.; Mandelli, L.; Mazzanti, M.; Meloni, F.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Rivoltella, G.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Vegni, G.; Volpini, G.] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Andreazza, A.; Besana, M. I.; Carminati, L.; Consonni, S. M.; Fanti, M.; Favareto, A.; Meloni, F.; Perini, L.; Pizio, C.; Ragusa, F.; Rivoltella, G.; Simoniello, R.; Turra, R.; Vegni, G.] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Satsounkevitch, I.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Banerjee, P.; Bouchami, J.; Davies, M.; Giunta, M.; Leroy, C.; Martin, J. P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.] Acad Sci, PN Lebedev Inst Phys, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.] Moscow Engn & Phys Inst MEPhI, Moscow, Russia. [Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Beale, S.; Becker, S.; Biebel, O.; Bortolotto, V.; Calfayan, P.; De Graat, J.; Duckeck, G.; Ebke, J.; Elmsheuser, J.; Engl, A.; Galea, C.; Heller, C.; Hertenberger, R.; Kummer, C.; Legger, F.; Lichtnecker, M.; Lorenz, J.; Mameghani, R.; Mueller, T. A.; Nunnemann, T.; Oakes, L. B.; Rauscher, F.; Reznicek, P.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Schieck, J.; Serfon, C.; Staude, A.; Vladoiu, D.; Walker, R.; Will, J. Z.; Zhuang, X.; Zibell, A.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Beimforde, M.; Bethke, S.; Bittner, B.; Bronner, J.; Capriotti, D.; Compostella, G.; Cortiana, G.; Dubbert, J.; Flowerdew, M. J.; Giovannini, P.; Ince, T.; Jantsch, A.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kotov, S.; Kroha, H.; Macchiolo, A.; Manfredini, A.; Menke, S.; Moser, H. G.; Nagel, M.; Nisius, R.; Oberlack, H.; Pahl, C.; Pospelov, G. E.; Potrap, I. N.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Stern, S.; Stonjek, S.; Vanadia, M.; Von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.; Zhuravlov, V.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Shimizu, S.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Shimizu, S.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Capasso, L.; Carlino, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; della Volpe, D.; Di Donato, C.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Musto, E.; Patricelli, S.; Sanchez, A.; Sekhniaidze, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Canale, V.; Capasso, L.; della Volpe, D.; Di Donato, C.; Giordano, R.; Merola, L.; Musto, E.; Patricelli, S.; Sanchez, A.] Univ Naples Federico II, Dipartimento Sci Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Chelstowska, M. A.; De Groot, N.; Filthaut, F.; Klok, P. F.; Koenig, A. C.; Koetsveld, F.; Raas, M.; Salvucci, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Boterenbrood, H.; Colijn, A. P.; De Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Doxiadis, A. D.; Ferrari, P.; Garitaonandia, H.; Geerts, D. A. A.; Gosselink, M.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kayl, M. S.; Klous, S.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Luijckx, G.; Mahlstedt, J.; Massaro, G.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Pani, P.; Rijpstra, M.; Ruckstuhl, N.; Ta, D.; Tsiakiris, M.; Turlay, E.; Van der Deijl, P. C.; Van der Geer, R.; Van der Graaf, H.; Van der Leeuw, R.; Van der Poel, E.; Van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Boterenbrood, H.; Colijn, A. P.; De Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Doxiadis, A. D.; Ferrari, P.; Garitaonandia, H.; Geerts, D. A. A.; Gosselink, M.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kayl, M. S.; Klous, S.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Luijckx, G.; Mahlstedt, J.; Massaro, G.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Pani, P.; Rijpstra, M.; Ruckstuhl, N.; Ta, D.; Tsiakiris, M.; Turlay, E.; Van der Deijl, P. C.; Van der Geer, R.; Van der Graaf, H.; Van der Leeuw, R.; Van der Poel, E.; Van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.] Univ Amsterdam, Amsterdam, Netherlands. [Calkins, R.; Chakraborty, D.; Cole, S.; De Lima, J. G. Rocha; Suhr, C.; Yurkewicz, A.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A.; Beloborodova, O.; Bobrovnikov, V. B.; Bogdanchikov, A.; Kazanin, V. A.; Kolachev, G. M.; Korol, A.; Malyshev, V.; Maslennikov, A. L.; Maximov, D. A.; Orlov, I.; Peleganchuk, S. V.; Schamov, A. G.; Skovpen, K.; Soukharev, A.; Talyshev, A.; Tikhonov, Y. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Budick, B.; Casadei, D.; Cranmer, K.; Haas, A.; Van Huysduynen, L. Hooft; Kaplan, B.; Konoplich, R.; Krasznahorkay, A.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.; Prokofiev, K.; Zhao, L.] NYU, Dept Phys, New York, NY 10003 USA. [Fisher, M. J.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Rahimi, A. M.; Strang, M.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Gutierrez, P.; Jana, D. K.; Marzin, A.; Meera-Lebbai, R.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Snow, J.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Khanov, A.; Rizatdinova, F.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Hamal, P.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Potter, C. T.; Ptacek, E.; Radloff, P.; Reinsch, A.; Searcy, J.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Andari, N.; Arnault, C.; Auge, E.; Barrillon, P.; Benoit, M.; Binet, S.; Bourdarios, C.; De la Taille, C.; De Regie, J. B. De Vivie; Dufiot, L.; Dueren, M.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Matricon, P.; Niedercorn, F.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Serif, L.; Simion, S.; Tanaka, R.; Teinturier, M.; Veillet, J. J.; Wicek, F.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Andari, N.; Arnault, C.; Auge, E.; Barrillon, P.; Benoit, M.; Binet, S.; Bourdarios, C.; De la Taille, C.; De Regie, J. B. De Vivie; Dufiot, L.; Dueren, M.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Matricon, P.; Niedercorn, F.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Serif, L.; Simion, S.; Tanaka, R.; Teinturier, M.; Veillet, J. J.; Wicek, F.; Zerwas, D.; Zhang, Z.] CNRS, IN2P3, F-91405 Orsay, France. [Hanagaki, K.; Hirose, M.; Lee, J. S. H.; Meguro, T.; Nomachi, M.; Okamura, W.; Sugaya, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Buran, T.; Cameron, D.; Gjelsten, B. K.; Gramstad, E.; Lund, E.; Ould-Saada, F.; Pajchel, K.; Read, A. L.; Rohne, O.; Samset, B. H.; Smestad, L.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Apolle, R.; Barr, A. J.; Boddy, C. R.; Brandt, G.; Buchanan, J.; Buckingham, R. M.; Cooper-Sarkar, A. M.; Dafinca, A.; Davies, E.; Gallas, E. J.; Gwenlan, C.; Hall, D.; Hays, C. P.; Howard, J.; Huffman, T. B.; Issever, C.; King, R. S. B.; Kogan, L. A.; Korn, A.; Larner, A.; Lewis, A.; Liang, Z.; Livermore, S. S. A.; Mattravers, C.; Nickerson, R. B.; Pinder, A.; Robichaud-Veronneau, A.; Ryder, N. C.; Short, D.; Tseng, J. C-L.; Vickey, T.; Viehhauser, G. H. A.; Weidberg, A. R.; Whitehead, S. R.; Young, C. J.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Colombo, T.; Conta, C.; Ferrari, R.; Franchino, S.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Uslenghi, M.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Colombo, T.; Conta, C.; Franchino, S.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.; Uslenghi, M.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Alison, J.; Brendlinger, K.; Degenhardt, J.; Dressnandt, N.; Fratina, S.; Heim, S. 120; Hines, E.; Hong, T. M.; Jackson, B.; Keener, P. T.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Newcomer, F. M.; Olivito, D.; Ospanov, R.; Reece, R.; Saxon, J.; Schaefer, D.; Stahlman, J.; Thomson, E.; Van Berg, R.; Wagner, P.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Bertolucci, F.; Cascella, M.; Cavasinni, V.; Crescioli, F.; Del Prete, T.; Dotti, A.; Roda, C.; Sarri, F.; White, S.; Zinonos, Z.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Bertolucci, F.; Cascella, M.; Cavasinni, V.; Crescioli, F.; Del Prete, T.; Dotti, A.; Roda, C.; Sarri, F.; White, S.; Zinonos, Z.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Boudreau, J.; Cleland, W.; Escobar, C.; Kittelmann, T.; Mueller, J.; Prieur, D.; Savinov, V.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Dos Santos, S. P. Amor; Amorim, A.; Anjos, N.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Wemans, A. Do Valle; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Jorge, P. M.; Lopes, L.; Miguens, J. Machado; Maio, A.; Mancira, J.; Oliveira, M.; Onofre, A.; Palma, A.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Gomes, A.; Maio, A.; Pina, J.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Amorim, A.; Gomes, A.; Maio, A.; Pina, J.] Univ Granada, CAFPE, Granada, Spain. [Bohm, J.; Chudoba, J.; Gallus, P.; Gunther, J.; Jakoubek, T.; Juranek, V.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Marcisovsky, M.; Mikestikova, M.; Myska, M.; Nemecek, S.; Ruzicka, P.; Schovancova, J.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Tic, T.; Valenta, J.; Vrba, V.; Zeman, M.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Balek, P.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Kodys, P.; Leitner, R.; Novakova, J.; Rybar, M.; Spousta, M.; Strachota, P.; Suk, M.; Sykora, T.; Tas, P.; Valkar, S.; Vorobel, V.; Wilhelm, I.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Augsten, K.; Holy, T.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Kral, V.; Krejci, F.; Pospisil, S.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solar, M.; Solc, J.; Sopko, V.; Sopko, B.; Stekl, I.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Ammosov, V. V.; Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Ivashin, A. V.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.; Zmouchko, V. V.] State Res Ctr Inst High Energy Phys, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Gillman, A. R.; Haywood, S. J.; Kirk, J.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Norton, P. R.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Benslama, K.; Smit, G. V. Ybeles] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anghinolfi, F.; Anulli, F.; Artoni, G.; Bagnaia, P.; Bini, C.; Caloi, R.; Chiefari, G.; Ciapetti, G.; D'Orazio, A.; De Pedis, D.; De Salvo, A.; De Zorzi, G.; Dionisi, C.; Falciano, S.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Rossi, E.; Tehrani, F. Safai; Sidoti, A.; Camillocci, E. Solfaroli; Vari, R.; Veneziano, S.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma 1, Rome, Italy. [Bini, C.; Caloi, R.; Chiefari, G.; Ciapetti, G.; D'Orazio, A.; De Zorzi, G.; Dionisi, C.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Messina, A.; Rossi, E.; Camillocci, E. Solfaroli; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Di Simone, A.; Liberti, B.; Marchese, F.; Mazzaferro, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Camarri, P.; Cattani, G.; Di Ciaccio, A.; Di Simone, A.; Mazzaferro, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Bos, K.; Branchini, P.; Ceradini, F.; Di Luise, S.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Stanescu, C.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bos, K.; Ceradini, F.; Di Luise, S.; Orestano, D.; Pastore, F.; Petrucci, F.] Univ Roma Tre, Dipartimento Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.; Lablak, S.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA Marrakech, Fac Sci Semlalia, Marrakech, Morocco. [Derkaoui, J. E.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui] Univ Mohammed VAgdal, Fac Sci, Rabat, Morocco. [Abreu, H.; Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Bolnet, N. M.; Boonekamp, M.; Chevalier, L.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Gauthier, L.; Giraud, P. F.; Guyot, C.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Legendre, M.; Maiani, C.; Mal, P.; Ramos, J. A. Manjarres; Mansoulie, B.; Meyer, J-P.; Mijovic, L.; Morange, N.; Mountricha, E.; Hong, V. Nguyen Thi; Nicolaidou, R.; Ouraou, A.; Resende, B.; Royon, C. R.; Schoeffel, L.; Schune, Ph.; Schwindling, J.; Simard, O.; Virchaux, M.; Vranjes, N.; Xiao, M.] CEA Saclay Commissariat Energie Atom, DSM IRFU Inst Rech Lois Fondamentales Univers, F-91191 Gif Sur Yvette, France. [Chouridou, S.; Damiani, D. S.; Grillo, A. A.; Hare, G. A.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Mitrevski, J.; Nielsen, J.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Beckingham, M.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Keller, J. S.; Lubatti, H. J.; Rompotis, N.; Rothberg, J.; Verducci, M.; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Duxfield, R.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Mayne, A.; Mcfayden, J. A.; Miyagawa, P. S.; Owen, S.; Paganis, E.; Suruliz, K.; Tovey, D. R.; Tsionou, D.; Tua, A.; Xu, D.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Holder, M.; Ibragimov, I.; Rammes, M.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Dawe, E.; Godfrey, J.; Kvita, J.; O'Neil, D. C.; Petteni, M.; Stelzer, B.; Tanasijczuk, A. J.; Trottier-McDonald, M.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Mayes, J. Backus; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Butler, B.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Grenier, P.; Hansson, P.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nelson, T. K.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Smith, D.; Strauss, E.; Su, D.; Wilson, M. G.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Batkova, L.; Blazek, T.; Federic, P.; Pecsy, M.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Ferencci, J.; Kladiva, E.; Seman, M.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Aurousseau, M.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Hamilton, A.; Leney, K. J. C.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Asman, B.; Bendtz, K.; Bohm, C.; Clement, C.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Holmgren, S. O.; Johansen, M.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Papadelis, A.; Sellden, B.; Silverstein, S. B.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Asman, B.; Bendtz, K.; Clement, C.; Gellerstedt, K.; Hellman, S.; Johansen, M.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Ahmad, A.; Arfaoui, S.; Devetak, E.; DeWilde, B.; Engelmann, R.; Farley, J.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Li, H.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Ahmad, A.; Arfaoui, S.; Devetak, E.; DeWilde, B.; Engelmann, R.; Farley, J.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Li, H.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Bartsch, V.; De Santo, A.; Martin-Haugh, S.; Potter, C. J.; Rose, A.; Salvatore, F.; Sutton, M. R.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Bangert, A.; Cuthbert, C.; Patel, N.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Waugh, A. T.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Chu, M. L.; Hou, S.; Jamin, D. O.; Lee, S. C.; Lin, S. C.; Liu, D.; Mazini, R.; Meng, Z.; Ren, Z. L.; Soh, D. A.; Teng, P. K.; Wang, H.; Wang, J.; Wang, S. M.; Weng, Z.; Zhang, D.; Zhou, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Harpaz, S. Behar; Kajomovitz, E.; Kopeliansky, R.; Rozen, Y.; Tarem, S.; Vallecorsa, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Bella, G.; Benary, O.; Benhammou, Y.; Etzion, E.; Gershon, A.; Ginzburg, J.; Guttman, N.; Hod, N.; Munwes, Y.; Oren, Y.; Reinherz-Aronis, E.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Iliadis, D.; Kordas, K.; Kouskoura, V.; Nomidis, I.; Petridis, A.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, K.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yamazaki, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, K.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yamazaki, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Ishitsuka, M.; Jinnouchi, O.; Kanno, T.; Kuze, M.; Nagai, R.; Nobe, T.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Bailey, D. C.; Bain, T.; Brelier, B.; Cheung, S. L.; Dhaliwal, S.; Farooque, T.; Fatholahzadeh, B.; Gibson, A.; Guo, B.; Ilic, N.; Keung, J.; Krieger, P.; Martens, F. K.; Orr, R. S.; Rezvani, R.; Rosenbaum, G. A.; Savard, P.; Sinervo, P.; Spreitzer, T.; Tardif, D.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Anisenkov, A.; Canepa, A.; Chekulaev, S. V.; Fortin, D.; Koutsmans, A.; Losty, M. J.; Nugent, I. M.; Oram, C. J.; Codina, E. Perez; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hanawa, K.; Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Kurata, M.; Nagai, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Napier, A.; Rolli, S.; Sliwa, K.; Todorova-Nova, S.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Loureiro, K. F.; Navas, L. Mendoza; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Deng, J.; Farrell, S.; Eschrich, I. Gough; Lankford, A. J.; Magnoni, L.; Mete, A. S.; Nelson, A.; Scannicchio, D. A.; Schernau, M.; Taffard, A.; Toggerson, B.; Unel, G.; Werth, M.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Del Papa, C.; Pinamonti, M.; Shaw, K.; Soualah, R.] Ist Nazl Fis Nucl, Grp Collegato Udine, Udine, Italy. [Acharya, B. S.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Alhroob, M.; Giordani, M. P.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Coggeshall, J.; Cortes-Gonzalez, A.; Errede, D.; Errede, S.; Lie, K.; Liss, T. M.; McCarn, A.; Neubauer, M. S.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Brenner, R.; Buszello, C. P.; Coniavitis, E.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Pelikan, D.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; De la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Martinez, V. Sanchez; Solans, C. A.; Soldevila, U.; Sanchez, J.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; De la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Martinez, V. Sanchez; Solans, C. A.; Soldevila, U.; Sanchez, J.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; De la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Martinez, V. Sanchez; Solans, C. A.; Soldevila, U.; Sanchez, J.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; De la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Martinez, V. Sanchez; Solans, C. A.; Soldevila, U.; Sanchez, J.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; De la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Martinez, V. Sanchez; Solans, C. A.; Soldevila, U.; Sanchez, J.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Perez, M. Villaplana; Vos, M.] CSIC, Valencia, Spain. [Axen, D.; Gay, C.; Gecse, Z.; Loh, C. W.; Mills, W. J.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Astbury, A.; Bansal, V.; Berghaus, F.; Courneyea, L.; Fincke-Keeler, M.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Lessard, J-R.; Marino, C. P.; Martyniuk, A. C.; McPherson, R. A.; Ouellette, E. A.; Plamondon, M.; Sobie, R.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Farrington, S. M.; Jones, G.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Kimura, N.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Alon, R.; Barak, L.; Bressler, S.; Citron, Z. H.; Duchovni, E.; Frank, T.; Gabizon, O.; Gross, E.; Groth-Jensen, J.; Klier, A.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Milstein, D.; Roth, I.; Silbert, O.; Smakhtin, V.; Vitells, O.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Carrillo-Montoya, G. D.; Hernandez, A. M. Castaneda; Castaneda-Miranda, E.; Chen, X.; Di Mattia, A.; Dos Anjos, A.; Fang, Y.; Castillo, L. R. Flores; Gutzwiller, O.; Ji, H.; Ju, X.; Kashif, L.; Ma, L. L.; Garcia, B. R. Mellado; Ming, Y.; Pan, Y. B.; Morales, M. I. Pedraza; Quayle, W. B.; Sarangi, T.; Wang, H.; Wiedenmann, W.; Wu, S. L.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Fleischmann, P.; Meyer, J.; Redelbach, A.; Siragusa, G.; Strohmer, R.; Trefzger, T.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Barisonzi, M.; Becker, A. K.; Becks, K. H.; Boek, J.; Braun, H. M.; Cornelissen, T.; Duda, D.; Fleischmann, S.; Flick, T.; Gerlach, P.; Glitza, K. W.; Gorfine, G.; Hamacher, K.; Harenberg, T.; Henss, T.; Hirschbuehl, D.; Kalinin, S.; Kersten, S.; Khoroshilov, A.; Kohlmann, S.; Lantzsch, K.; Lenzen, G.; Mattig, P.; Mechtel, M.; Neumann, M.; Pataraia, S.; Sandhoff, M.; Sartisohn, G.; Schultes, J.; Sturm, P.; Voss, T. T.; Wagner, W.; Wahlen, H.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany. [Adelman, J.; Baker, O. K.; Bedikian, S.; Almenar, C. Cuenca; Czyczula, Z.; Demers, S.; Garberson, F.; Golling, T.; Guest, D.; Henrichs, A.; Lagouri, T.; Lee, L.; Loginov, A.; Sherman, D.; Tipton, P.; Wall, R.; Walsh, B.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Biscarat, C.; Cogneras, E.; Rahal, G.] Ctr Calcul, Inst Natl Phys Nucl & Phys Particules IN2P3, Villeurbanne, France. Univ Lisbon, Fac Ciencias, Lisbon, Portugal. Univ Lisbon, CFNUL, Lisbon, Portugal. 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C.] Acad Sinica, Acad Sinica Grid Comp, Inst Phys, Taipei 115, Taiwan. [Meng, Z.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Park, W.; Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Pasztor, G.; Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. CALTECH, Pasadena, CA 91125 USA. [Richter-Was, E.] Jagiellonian Univ, Inst Phys, Krakow, Poland. [Ruan, X.] Univ Paris 11, LAL, Orsay, France. [Ruan, X.] CNRS, IN2P3, F-91405 Orsay, France. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. RP Aad, G (reprint author), Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. 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Nemecek, Stanislav/G-5931-2014; Kepka, Oldrich/G-6375-2014; Lokajicek, Milos/G-7800-2014; Jakoubek, Tomas/G-8644-2014; Boyko, Igor/J-3659-2013; Kuleshov, Sergey/D-9940-2013; Anjos, Nuno/I-3918-2013; Kartvelishvili, Vakhtang/K-2312-2013; Prokoshin, Fedor/E-2795-2012; Dawson, Ian/K-6090-2013; Ferrando, James/A-9192-2012; Tudorache, Valentina/D-2743-2012; Marti-Garcia, Salvador/F-3085-2011; Castro, Nuno/D-5260-2011; Wolters, Helmut/M-4154-2013; Brooks, William/C-8636-2013; Stoicea, Gabriel/B-6717-2011; Doyle, Anthony/C-5889-2009; Pina, Joao /C-4391-2012; Amorim, Antonio/C-8460-2013; Solfaroli Camillocci, Elena/J-1596-2012; Vanyashin, Aleksandr/H-7796-2013; Moorhead, Gareth/B-6634-2009; Casadei, Diego/I-1785-2013; La Rosa, Alessandro/I-1856-2013; Moraes, Arthur/F-6478-2010; Smirnov, Sergei/F-1014-2011; Conde Muino, Patricia/F-7696-2011; Andreazza, Attilio/E-5642-2011; Grancagnolo, Sergio/J-3957-2015; spagnolo, stefania/A-6359-2012; Shmeleva, Alevtina/M-6199-2015; Camarri, Paolo/M-7979-2015; Gavrilenko, Igor/M-8260-2015; Tikhomirov, Vladimir/M-6194-2015; Chekulaev, Sergey/O-1145-2015; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; Carvalho, Joao/M-4060-2013; Mashinistov, Ruslan/M-8356-2015; Gonzalez de la Hoz, Santiago/E-2494-2016; Fassi, Farida/F-3571-2016; la rotonda, laura/B-4028-2016; Karyukhin, Andrey/J-3904-2014; Capua, Marcella/A-8549-2015; Tartarelli, Giuseppe Francesco/A-5629-2016; KHODINOV, ALEKSANDR/D-6269-2015; Goncalo, Ricardo/M-3153-2016; Gauzzi, Paolo/D-2615-2009; O'Shea, Val/G-1279-2010; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Yang, Haijun/O-1055-2015; Monzani, Simone/D-6328-2017; Grancagnolo, Francesco/K-2857-2015; Korol, Aleksandr/A-6244-2014; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Wemans, Andre/A-6738-2012; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Olshevskiy, Alexander/I-1580-2016; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Mora Herrera, Maria Clemencia/L-3893-2016 OI Ventura, Andrea/0000-0002-3368-3413; Livan, Michele/0000-0002-5877-0062; Mitsou, Vasiliki/0000-0002-1533-8886; Joergensen, Morten/0000-0002-6790-9361; Mir, Lluisa-Maria/0000-0002-4276-715X; Riu, Imma/0000-0002-3742-4582; Della Pietra, Massimo/0000-0003-4446-3368; Petrucci, Fabrizio/0000-0002-5278-2206; Negrini, Matteo/0000-0003-0101-6963; Ferrer, Antonio/0000-0003-0532-711X; Hansen, John/0000-0002-8422-5543; Mikestikova, Marcela/0000-0003-1277-2596; Kuday, Sinan/0000-0002-0116-5494; Tomasek, Lukas/0000-0002-5224-1936; Svatos, Michal/0000-0002-7199-3383; Peleganchuk, Sergey/0000-0003-0907-7592; Santamarina Rios, Cibran/0000-0002-9810-1816; Bosman, Martine/0000-0002-7290-643X; Warburton, Andreas/0000-0002-2298-7315; De, Kaushik/0000-0002-5647-4489; Lee, Jason/0000-0002-2153-1519; Smirnova, Oxana/0000-0003-2517-531X; Fabbri, Laura/0000-0002-4002-8353; Villa, Mauro/0000-0002-9181-8048; Boyko, Igor/0000-0002-3355-4662; Kuleshov, Sergey/0000-0002-3065-326X; Prokoshin, Fedor/0000-0001-6389-5399; Ferrando, James/0000-0002-1007-7816; Castro, Nuno/0000-0001-8491-4376; Wolters, Helmut/0000-0002-9588-1773; Brooks, William/0000-0001-6161-3570; Stoicea, Gabriel/0000-0002-7511-4614; Doyle, Anthony/0000-0001-6322-6195; Pina, Joao /0000-0001-8959-5044; Solfaroli Camillocci, Elena/0000-0002-5347-7764; Vanyashin, Aleksandr/0000-0002-0367-5666; Moorhead, Gareth/0000-0002-9299-9549; La Rosa, Alessandro/0000-0001-6291-2142; Moraes, Arthur/0000-0002-5157-5686; Smirnov, Sergei/0000-0002-6778-073X; Conde Muino, Patricia/0000-0002-9187-7478; Andreazza, Attilio/0000-0001-5161-5759; Grancagnolo, Sergio/0000-0001-8490-8304; spagnolo, stefania/0000-0001-7482-6348; Camarri, Paolo/0000-0002-5732-5645; Tikhomirov, Vladimir/0000-0002-9634-0581; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; Carvalho, Joao/0000-0002-3015-7821; Mashinistov, Ruslan/0000-0001-7925-4676; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Veloso, Filipe/0000-0002-5956-4244; Gomes, Agostinho/0000-0002-5940-9893; Fassi, Farida/0000-0002-6423-7213; la rotonda, laura/0000-0002-6780-5829; Osculati, Bianca Maria/0000-0002-7246-060X; Amorim, Antonio/0000-0003-0638-2321; Santos, Helena/0000-0003-1710-9291; Coccaro, Andrea/0000-0003-2368-4559; Maio, Amelia/0000-0001-9099-0009; Fiolhais, Miguel/0000-0001-9035-0335; Karyukhin, Andrey/0000-0001-9087-4315; Anjos, Nuno/0000-0002-0018-0633; Smestad, Lillian/0000-0002-0244-8736; Giordani, Mario/0000-0002-0792-6039; Abdelalim, Ahmed Ali/0000-0002-2056-7894; Capua, Marcella/0000-0002-2443-6525; Di Micco, Biagio/0000-0002-4067-1592; Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; Doria, Alessandra/0000-0002-5381-2649; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Goncalo, Ricardo/0000-0002-3826-3442; Gauzzi, Paolo/0000-0003-4841-5822; O'Shea, Val/0000-0001-7183-1205; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Monzani, Simone/0000-0002-0479-2207; Grancagnolo, Francesco/0000-0002-9367-3380; Korol, Aleksandr/0000-0001-8448-218X; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Wemans, Andre/0000-0002-9669-9500; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Olshevskiy, Alexander/0000-0002-8902-1793; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Mora Herrera, Maria Clemencia/0000-0003-3915-3170 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union; ERC, European Union; IN2P3-CNRS, France; CEADSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; ISF, Israel; MINERVA, Israel; GIF, Israel; DIP, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; GRICES, Portugal; FCT, Portugal; MERYS (MECTS), Romania; MES of Russia; ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MVZT, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET and ERC, European Union; IN2P3-CNRS, CEADSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT, Greece; ISF, MINERVA, GIF, DIP and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW, Poland; GRICES and FCT, Portugal; MERYS (MECTS), Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MVZT, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. NR 34 TC 23 Z9 23 U1 6 U2 125 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 J9 EUR PHYS J C JI Eur. Phys. J. C PD JAN PY 2013 VL 73 IS 1 AR 2263 DI 10.1140/epjc/s10052-012-2263-z PG 20 WC Physics, Particles & Fields SC Physics GA 135KX UT WOS:000318288100004 ER PT J AU Rose, LS Levinson, R AF Rose, L. Shea Levinson, Ronnen TI Analysis of the effect of vegetation on albedo in residential areas: case studies in suburban Sacramento and Los Angeles, CA SO GISCIENCE & REMOTE SENSING LA English DT Article DE urban fabric; albedo; urban greening; albedo; vegetation; sustainability; urban LULC; GIS ID DIGITAL ORTHOPHOTOGRAPHY; LAND-COVER; URBAN; LANDSCAPE AB Increasingly "urban greening" is being implemented in order to meet goals of sustainability. Tree planting is part of these efforts that provide climate and environmental benefits. Albedo is an important factor in climatological and ecological functioning. Using GIS, this study assesses albedo changes of suburban communities resulting from trees. Based on orthophotos and LiDAR, a shading algorithm is used to examine how tree shading changes albedo throughout the year. For comparison, changes in community albedo were calculated with low and high assumptions for tree albedo. Under the low tree albedo assumption (0.14), community albedo was decreased (-0.07) by the effect of tree shading at all times modeled during the year. Using a high albedo for trees (0.20), the albedo changes were slight (<-0.01). This indicates the importance of considering the albedo of both the trees planted and the surfaces that are shaded when developing urban greening policies. C1 [Rose, L. Shea] Univ West Georgia, Dept Geosci, Carrollton, GA 30118 USA. [Levinson, Ronnen] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Heat Isl Grp, Berkeley, CA 94720 USA. RP Rose, LS (reprint author), Univ West Georgia, Dept Geosci, 1601 Maple St, Carrollton, GA 30118 USA. EM srose@westga.edu FU California Energy Commission (CEC) through its Public Interest Energy Research Program (PIER); Office of Building Technology, State, and Community Programs, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the California Energy Commission (CEC) through its Public Interest Energy Research Program (PIER). It was also supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Building Technology, State, and Community Programs, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The students at the University of West Georgia were invaluable to the immense digitizing effort in support of this project. The author is grateful for the efforts of Zach Little, David Finni, Jon Indridason, and Sean Bickell. NR 26 TC 2 Z9 2 U1 1 U2 22 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND SN 1548-1603 J9 GISCI REMOTE SENS JI GISci. Remote Sens. PY 2013 VL 50 IS 1 BP 64 EP 77 DI 10.1080/15481603.2013.778557 PG 14 WC Geography, Physical; Remote Sensing SC Physical Geography; Remote Sensing GA 139PP UT WOS:000318596200004 ER PT S AU Awwal, AAS Orth, C Tse, E Matone, J Paul, M Hardy, C Brunton, G Hermann, M Yang, S DiNicola, JM Rever, M Dixit, S Heebner, J AF Awwal, Abdul A. S. Orth, Charles Tse, Eddy Matone, JoAnn Paul, Mitanu Hardy, Carla Brunton, Gordon Hermann, Mark Yang, Steve DiNicola, J. M. Rever, Matt Dixit, Sham Heebner, John BE Awwal, AAS TI Image processing and control of a programmable spatial light modulator for spatial beam shaping SO HIGH POWER LASERS FOR FUSION RESEARCH II SE Proceedings of SPIE LA English DT Proceedings Paper CT Conference on High Power Lasers for Fusion Research II CY FEB 07, 2013 CL San Francisco, CA SP SPIE, NIF DE control systems; laser alignment; beam shaping; liquid crystal device; spatial light modulator ID NATIONAL-IGNITION-FACILITY; AUTOMATIC ALIGNMENT; LASER AB Programmable spatial shapers using liquid-crystal-based spatial-light-modulators in the National Ignition Facility lasers enable spatial shaping of the beam profile so that power delivered to the target can be maximized while maintaining system longevity. Programmable spatial shapers achieve three objectives: Introduce obscurations shadowing isolated flaws on downstream optical elements that could otherwise be affected by high fluence laser illumination; Spatial shaping to reduce beam peak-to-mean fluence variations to allow the laser to operate at higher powers so that maximum power can be delivered to the target; And finally gradually exposing the optical regions that have never seen laser light because they have always had shadowing from a blocker that is no longer needed. In this paper, we describe the control and image processing algorithms that determine beam shaping and verification of the beam profile. Calibration and transmittance mapping essential elements of controlling the PSS are described along with spatially nonlinear response of the device such as scale and rotation. C1 [Awwal, Abdul A. S.; Orth, Charles; Tse, Eddy; Matone, JoAnn; Paul, Mitanu; Hardy, Carla; Brunton, Gordon; Hermann, Mark; Yang, Steve; DiNicola, J. M.; Rever, Matt; Dixit, Sham; Heebner, John] Lawrence Livermore Natl Lab, Comp Engn Div, Natl Ignit Facil, Integrated Comp Control Syst, Livermore, CA 94551 USA. RP Awwal, AAS (reprint author), Lawrence Livermore Natl Lab, Comp Engn Div, Natl Ignit Facil, Integrated Comp Control Syst, Livermore, CA 94551 USA. EM awwal1@llnl.gov NR 19 TC 3 Z9 3 U1 0 U2 5 PU SPIE-INT SOC OPTICAL ENGINEERING PI BELLINGHAM PA 1000 20TH ST, PO BOX 10, BELLINGHAM, WA 98227-0010 USA SN 0277-786X BN 978-0-8194-9371-2 J9 PROC SPIE PY 2013 VL 8602 AR 86020A DI 10.1117/12.2008542 PG 12 WC Optics; Physics, Fluids & Plasmas SC Optics; Physics GA BEX24 UT WOS:000318517700006 ER PT S AU Burkhart, SC Awwal, A Borden, M Budge, T Campbell, J Dixit, S Henesian, M Jancaitis, K Jedlovec, D Leach, R Lowe-Webb, R MacGowan, B Pratuch, S Palma, J Salmon, T Smauley, D Smith, L Sommer, S Wegner, P Wilhelmsen, K Witte, M Wong, N AF Burkhart, S. C. Awwal, A. Borden, M. Budge, T. Campbell, J. Dixit, S. Henesian, M. Jancaitis, K. Jedlovec, D. Leach, R. Lowe-Webb, R. MacGowan, B. Pratuch, S. Palma, J. Salmon, T. Smauley, D. Smith, L. Sommer, S. Wegner, P. Wilhelmsen, K. Witte, M. Wong, N. BE Awwal, AAS TI The National Ignition Facility - Beam Area Increase SO HIGH POWER LASERS FOR FUSION RESEARCH II SE Proceedings of SPIE LA English DT Proceedings Paper CT Conference on High Power Lasers for Fusion Research II CY FEB 07, 2013 CL San Francisco, CA SP SPIE, NIF ID LINE-REPLACEABLE UNITS; AUTOMATIC ALIGNMENT; LASER AB he National Ignition Facility (NIF) is the world's most energetic laser, having demonstrated in excess of 1.9MJ @351nm with Inertial Confinement Fusion pulse-shapes in July, 2012. First commissioned with 192 operational beamlines in March, 2009, NIF has since transitioned to routine operation for stockpile stewardship, inertial confinement fusion research, and basic high energy density science. The NIF design includes component placement and beam alignment tolerances to preclude laser beam clipping on components within the laser chain, indeed lengthy studies and analyses, including various statistical approaches, were done in the design phase as early as 1996. The margin between the available optical aperture and the beam was established to ensure, given beam centering variations and component placement errors, that we would achieve a confidence level such that even low-level clipping, which causes downstream modulation damage, would occur at an acceptably or even vanishingly low rate. With the completion of NIF and nearly 4 years of operational experience, it became apparent that we could increase the beam size to more optimally fill the available aperture, and gain an additional 5% to 10% or more energy and power delivered to targets. It was also shown that additional energy could be recovered by removing approximately 70% of our beam 'corner blockers' originally installed in May 2010 to prevent target-chamber 1 mu m counterpropagating light from leaking back through the extinction minimums at the corners of vacuum-loaded square optics. Subsequent analyses showed that only one and in some cases two of the corner blockers were really needed. Increasing the beam size was a challenging endeavor, however, as it fundamentally meant recommissioning the entire NIF laser chain to tailor all 192 beams to their specific available aperture, individual beam rotation (for the NIF square beam), beam centering offsets, change-out of the 48 front-end aperture (relay-plane "0"), and removal of 48 Laser Mirror #2 line replaceable units for corner-blocker removal. Some of this commissioning, such as tailoring beam sizes to their specific available aperture, had not been performed during the original commissioning. Furthermore, achieving this required precise diagnostics and rapid analysis of massive quantities of images and data in order to direct the changes and feed-back the achieved results. Completed on June 1, 2012, the beam area was increased by 7.5%, and was a significant contributing factor in NIF transitioning from a 1.6MJ laser to its present 1.9MJ capability C1 [Burkhart, S. C.; Awwal, A.; Borden, M.; Budge, T.; Campbell, J.; Dixit, S.; Henesian, M.; Jancaitis, K.; Jedlovec, D.; Leach, R.; Lowe-Webb, R.; MacGowan, B.; Pratuch, S.; Palma, J.; Salmon, T.; Smauley, D.; Smith, L.; Sommer, S.; Wegner, P.; Wilhelmsen, K.; Witte, M.; Wong, N.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RP Burkhart, SC (reprint author), Lawrence Livermore Natl Lab, POB 808, Livermore, CA 94551 USA. NR 13 TC 0 Z9 0 U1 1 U2 5 PU SPIE-INT SOC OPTICAL ENGINEERING PI BELLINGHAM PA 1000 20TH ST, PO BOX 10, BELLINGHAM, WA 98227-0010 USA SN 0277-786X BN 978-0-8194-9371-2 J9 PROC SPIE PY 2013 VL 8602 AR 860203 DI 10.1117/12.2009402 PG 13 WC Optics; Physics, Fluids & Plasmas SC Optics; Physics GA BEX24 UT WOS:000318517700001 ER PT S AU Labaria, GR Liebman, JA Sayre, DB Herrmann, HW Bond, EJ Church, JA AF Labaria, George R. Liebman, Judith A. Sayre, Daniel B. Herrmann, Hans W. Bond, Essex J. Church, Jennifer A. BE Awwal, AAS TI Multi-objective optimization for the National Ignition Facility's Gamma Reaction History diagnostic SO HIGH POWER LASERS FOR FUSION RESEARCH II SE Proceedings of SPIE LA English DT Proceedings Paper CT Conference on High Power Lasers for Fusion Research II CY FEB 07, 2013 CL San Francisco, CA SP SPIE, NIF DE multi-objective; optimization; gamma-ray reaction history AB The National Ignition Facility (NIF) is producing experimental results for the study of Inertial Confinement Fusion (ICF) . The Gamma Reaction History (GRH) diagnostic at NIF can detect gamma rays to measure fusion burn parameters such as fusion burn width, bang time, neutron yield, and areal density of the compressed ablator for cryogenic deuterium-tritium (DT) implosions. Gamma-ray signals detected with this diagnostic are inherently distorted by hardware impulse response functions (IRFs) and gains, and are comprised of several components including gamma rays from laser-plasma interactions (LPI) . One method for removing hardware distortions to approximate the gamma-ray reaction history is deconvolution. However, deconvolution of the distorted signal to obtain the gamma-ray reaction history and its associated parameters presents an ill-posed inverse problem and does not separate out the source components of the gamma-ray signal. A multi-dimensional parameter space model for the distorted gamma-ray signal has been developed in the literature. To complement a deconvolution, we develop a multi-objective optimization algorithm to determine the model parameters so that the error between the model and the collected gamma-ray data is minimized in the least-squares sense. The implementation of the optimization algorithm must be sufficiently robust to be used in automated production software. To achieve this level of robustness, impulse response signals must be carefully processed and constraints on the parameter space based on theory and experimentation must be implemented to ensure proper convergence of the algorithm. In this paper, we focus on the optimization algorithm's theory and implementation. C1 [Labaria, George R.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Labaria, George R.; Liebman, Judith A.; Sayre, Daniel B.; Bond, Essex J.; Church, Jennifer A.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Herrmann, Hans W.] Los Alamos Natl Lab, Los Alamos, NM USA. RP Labaria, GR (reprint author), Univ Calif Berkeley, Berkeley, CA 94720 USA. EM labaria.george@berkeley.edu; liebman1@llnl.gov FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52- 07NA27344, LLNL-CONF-611632] FX We thank the members of the GRH team for their useful discussions. This work performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52- 07NA27344. LLNL-CONF-611632 NR 7 TC 1 Z9 1 U1 3 U2 7 PU SPIE-INT SOC OPTICAL ENGINEERING PI BELLINGHAM PA 1000 20TH ST, PO BOX 10, BELLINGHAM, WA 98227-0010 USA SN 0277-786X BN 978-0-8194-9371-2 J9 PROC SPIE PY 2013 VL 8602 AR UNSP 86020C DI 10.1117/12.2009047 PG 12 WC Optics; Physics, Fluids & Plasmas SC Optics; Physics GA BEX24 UT WOS:000318517700007 ER PT S AU Leach, RR Field, JE Kegelmeyer, LM Kozioziemski, B Lee, T Mapoles, E Roberts, R Dylla-Spears, RJ Suratwala, T AF Leach, Richard R., Jr. Field, John E. Kegelmeyer, Laura Mascio Kozioziemski, Bernard Lee, Tanza Mapoles, Evan Roberts, Randy Dylla-Spears, Rebecca J. Suratwala, Tayyab BE Awwal, AAS TI Image processing methods for characterizing cryogenic target quality during fuel layer formation at the National Ignition Facility (NIF) SO HIGH POWER LASERS FOR FUSION RESEARCH II SE Proceedings of SPIE LA English DT Proceedings Paper CT Conference on High Power Lasers for Fusion Research II CY FEB 07, 2013 CL San Francisco, CA SP SPIE, NIF DE NIF; cryogenic hydrogen crystal growth; registration; symmetry; texture; image entropy; trend analysis; montage; seed formation; eigenimages ID INERTIAL CONFINEMENT FUSION AB A challenging aspect of preparing cryogenic targets for National Ignition Facility (NIF) ignition experiments is growing a single crystal layer (similar to 70 mu m thick) of solid frozen deuterium-tritium (DT) fuel on the inner surface of a spherical hollow plastic capsule 2 mm in diameter. For the most critical fusion experiments, the layer must be smooth, having uniform thickness, and largely free of isolated defects (e. g. grooves). A single target layer typically takes up to 18 hours to form. X-ray images on 3 orthogonal axes are used to monitor the growth of the crystal and evaluate the quality of the layer. While these methods provide a good indicator of target layer condition, new metrics are currently being developed to take advantage of other properties in the x-ray image, which may give earlier indications of target quality. These properties include symmetry of texture, seed formation, and eigenimage analysis. We describe the approach and associated image processing to evaluate and classify these metrics, whose goal is to improve overall layer production and better quantify the quality of the layer during its growth. C1 [Leach, Richard R., Jr.; Field, John E.; Kegelmeyer, Laura Mascio; Kozioziemski, Bernard; Lee, Tanza; Mapoles, Evan; Roberts, Randy; Dylla-Spears, Rebecca J.; Suratwala, Tayyab] Lawrence Livermore Natl Lab, Natl Ignit Facil, Natl Ignit Campaign, Livermore, CA 94551 USA. RP Leach, RR (reprint author), Lawrence Livermore Natl Lab, Natl Ignit Facil, Natl Ignit Campaign, Livermore, CA 94551 USA. EM leach1@llnl.gov NR 16 TC 0 Z9 0 U1 1 U2 6 PU SPIE-INT SOC OPTICAL ENGINEERING PI BELLINGHAM PA 1000 20TH ST, PO BOX 10, BELLINGHAM, WA 98227-0010 USA SN 0277-786X BN 978-0-8194-9371-2 J9 PROC SPIE PY 2013 VL 8602 AR 86020H DI 10.1117/12.2009413 PG 11 WC Optics; Physics, Fluids & Plasmas SC Optics; Physics GA BEX24 UT WOS:000318517700012 ER PT J AU Friedman, P Ball, R Beene, J Benhammou, Y Ben-Moshe, M Bentefour, H Chapman, JW Etzion, E Ferretti, C Levin, D Silver, Y Varner, R Weaverdyck, C Zhou, B AF Friedman, Peter Ball, Robert Beene, James Benhammou, Yan Ben-Moshe, Meny Bentefour, Hassan Chapman, J. W. Etzion, Erez Ferretti, Claudio Levin, Daniel Silver, Yiftah Varner, Robert Weaverdyck, Curtis Zhou, Bing TI Plasma panel-based radiation detectors SO JOURNAL OF THE SOCIETY FOR INFORMATION DISPLAY LA English DT Article DE plasma panel sensor; PPS; plasma panel radiation detector; plasma panel detector ID SIMULATION AB The plasma panel sensor (PPS) is a gaseous micropattern radiation detector under current development. It has many operational and fabrication principles common to plasma display panels. It comprises a dense matrix of small, gas plasma discharge cells within a hermetically sealed panel. As in plasma display panels, it uses nonreactive, intrinsically radiation-hard materials such as glass substrates, refractory metal electrodes, and mostly inert gas mixtures. We are developing these devices primarily as thin, low-mass detectors with gas gaps from a few hundred microns to a few millimeters. The PPS is a high gain, inherently digital device with the potential for fast response times, fine position resolution (<50-mu m RMS) and low cost. In this paper, we report on prototype PPS experimental results in detecting betas, protons, and cosmic muons, and we extrapolate on the PPS potential for applications including the detection of alphas, heavy ions at low-to-medium energy, thermal neutrons, and X-rays. C1 [Friedman, Peter] Integrated Sensors LLC, Ottawa Hills, OH 43606 USA. [Ball, Robert; Chapman, J. W.; Ferretti, Claudio; Levin, Daniel; Weaverdyck, Curtis; Zhou, Bing] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Benhammou, Yan; Ben-Moshe, Meny; Etzion, Erez; Silver, Yiftah] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Beene, James; Varner, Robert] Oak Ridge Natl Lab, Holifield Radioact Ion Beam Facil, Oak Ridge, TN USA. [Bentefour, Hassan] Ion Beam Applicat SA IBA, Louvain, Belgium. RP Friedman, P (reprint author), Integrated Sensors LLC, 2403 Evergreen Rd, Ottawa Hills, OH 43606 USA. EM peter@isensors.net FU US Department of Energy [DE-FG02-07ER84749, DE-SC0006204, DE-SC0006219, DE-FG02-12ER41788]; Office of Nuclear Physics at the US Department of Energy; United States-Israel Binational Science Foundation [2008123] FX This work was supported in part by the US Department of Energy under grant numbers DE-FG02-07ER84749, DE-SC0006204, DE-SC0006219, and DE-FG02-12ER41788. This work was also partially supported by the Office of Nuclear Physics at the US Department of Energy and the United States-Israel Binational Science Foundation under grant number 2008123. NR 8 TC 1 Z9 1 U1 1 U2 5 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1071-0922 J9 J SOC INF DISPLAY JI J. Soc. Inf. Disp. PD JAN PY 2013 VL 21 IS 1 BP 46 EP 54 DI 10.1002/jsid.151 PG 9 WC Engineering, Electrical & Electronic; Materials Science, Multidisciplinary; Optics; Physics, Applied SC Engineering; Materials Science; Optics; Physics GA 142MY UT WOS:000318802700009 ER PT J AU Kim, YM Schmidt, BJ Kidwai, AS Jones, MB Kaiser, BLD Brewer, HM Mitchell, HD Palsson, BO McDermott, JE Heffron, F Smith, RD Peterson, SN Ansong, C Hyduke, DR Metz, TO Adkins, JN AF Kim, Young-Mo Schmidt, Brian J. Kidwai, Afshan S. Jones, Marcus B. Kaiser, Brooke L. Deatherage Brewer, Heather M. Mitchell, Hugh D. Palsson, Bernhard O. McDermott, Jason E. Heffron, Fred Smith, Richard D. Peterson, Scott N. Ansong, Charles Hyduke, Daniel R. Metz, Thomas O. Adkins, Joshua N. TI Salmonella modulates metabolism during growth under conditions that induce expression of virulence genes SO MOLECULAR BIOSYSTEMS LA English DT Article ID ENTERICA SEROVAR TYPHIMURIUM; PROTEOMIC ANALYSIS; INTRACELLULAR SURVIVAL; INTERACTION NETWORKS; MASS-SPECTROMETRY; ESCHERICHIA-COLI; UNITED-STATES; OMICS DATA; METABOLOMICS; MODELS AB Salmonella enterica serovar Typhimurium (S. Typhimurium) is a facultative pathogen that uses complex mechanisms to invade and proliferate within mammalian host cells. To investigate possible contributions of metabolic processes to virulence in S. Typhimurium grown under conditions known to induce expression of virulence genes, we used a metabolomics-driven systems biology approach coupled with genome-scale modeling. First, we identified distinct metabolite profiles associated with bacteria grown in either rich or virulence-inducing media and report the most comprehensive coverage of the S. Typhimurium metabolome to date. Second, we applied an omics-informed genome-scale modeling analysis of the functional consequences of adaptive alterations in S. Typhimurium metabolism during growth under our conditions. Modeling efforts highlighted a decreased cellular capability to both produce and utilize intracellular amino acids during stationary phase culture in virulence conditions, despite significant abundance increases for these molecules as observed by our metabolomics measurements. Furthermore, analyses of omics data in the context of the metabolic model indicated rewiring of the metabolic network to support pathways associated with virulence. For example, cellular concentrations of polyamines were perturbed, as well as the predicted capacity for secretion and uptake. C1 [Kim, Young-Mo; Kaiser, Brooke L. Deatherage; Mitchell, Hugh D.; McDermott, Jason E.; Smith, Richard D.; Ansong, Charles; Metz, Thomas O.; Adkins, Joshua N.] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. [Schmidt, Brian J.; Palsson, Bernhard O.; Hyduke, Daniel R.] Univ Calif San Diego, Dept Bioengn, La Jolla, CA 92093 USA. [Kidwai, Afshan S.; Heffron, Fred] Oregon Hlth & Sci Univ, Dept Mol Microbiol & Immunol, Portland, OR 97239 USA. [Jones, Marcus B.; Peterson, Scott N.] J Craig Venter Inst, Rockville, MD 20850 USA. [Brewer, Heather M.] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. RP Metz, TO (reprint author), Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. EM thomas.metz@pnnl.gov; joshua.Adkins@pnnl.gov RI Smith, Richard/J-3664-2012; Kim, Young-Mo/D-3282-2009; OI Smith, Richard/0000-0002-2381-2349; Kim, Young-Mo/0000-0002-8972-7593; Adkins, Joshua/0000-0003-0399-0700; Metz, Tom/0000-0001-6049-3968 FU National Institute of Allergy and Infectious Diseases [Y1-AI-8401]; San Diego Center for Systems Biology; NIH/NIGMS [GM085764]; Department of Energy's (DOE) Office of Biological and Environmental Research; DOE [DE-AC05-76RLO 1830] FX This work was funded by the National Institute of Allergy and Infectious Diseases under Interagency agreement Y1-AI-8401. DRH is supported in part by a Seed Award from the San Diego Center for Systems Biology funded by NIH/NIGMS (GM085764). Significant portions of the work were performed at the Environmental Molecular Sciences Laboratory, a national scientific user facility sponsored by the Department of Energy's (DOE) Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory (PNNL) in Richland, Washington. PNNL is amulti-program national laboratory operated by Battelle for the DOE under Contract DE-AC05-76RLO 1830. NR 79 TC 17 Z9 18 U1 1 U2 26 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1742-206X EI 1742-2051 J9 MOL BIOSYST JI Mol. Biosyst. PY 2013 VL 9 IS 6 BP 1522 EP 1534 DI 10.1039/c3mb25598k PG 13 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA 139BS UT WOS:000318557100044 PM 23559334 ER PT J AU Liao, T Sun, CH Sun, ZQ Du, AJ Smith, S AF Liao, Ting Sun, Chenghua Sun, Ziqi Du, Aijun Smith, Sean TI Chemically modified ribbon edge stimulated H-2 dissociation: a first-principles computational study SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID DENSITY-FUNCTIONAL THEORY; MAGNETIC-PROPERTIES; HYDROGEN STORAGE; CARBON NANOTUBES; METAL-CATALYSTS; SURFACE; OXIDE; DESORPTION; MONOLAYERS; MECHANISM AB First-principles computational studies indicate that (B, N, or O)-doped graphene ribbon edges can substantially reduce the energy barrier for H-2 dissociative adsorption. The low barrier is competitive with many widely used metal or metal oxide catalysts. This suggests that suitably functionalized graphene architectures are promising metal-free alternatives for low-cost catalytic processes. C1 [Liao, Ting; Sun, Chenghua; Du, Aijun] Univ Queensland, Australian Inst Bioengn & Nanotechnol, Computat Bio & Nanotechnol Grp, Brisbane, Qld 4072, Australia. [Sun, Chenghua] Univ Queensland, Australian Inst Bioengn & Nanotechnol, ARC Ctr Excellence Funct Nanomat, Brisbane, Qld 4072, Australia. [Sun, Ziqi] Univ Wollongong, Inst Superconducting & Elect Mat, Wollongong, NSW 2500, Australia. [Smith, Sean] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Liao, T (reprint author), Univ Queensland, Australian Inst Bioengn & Nanotechnol, Computat Bio & Nanotechnol Grp, Brisbane, Qld 4072, Australia. EM t.liao1@uq.edu.au; smithsc@ornl.gov RI Sun, Ziqi/A-8122-2011; Sun, Chenghua/C-5734-2009; LIAO, Ting/C-7027-2012; Du, Aijun/C-5759-2009 OI Sun, Ziqi/0000-0002-4777-4017; LIAO, Ting/0000-0001-7488-6244; Du, Aijun/0000-0002-3369-3283 NR 32 TC 10 Z9 10 U1 3 U2 32 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PY 2013 VL 15 IS 21 BP 8054 EP 8057 DI 10.1039/c3cp50654a PG 4 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 139EV UT WOS:000318565500013 PM 23632601 ER PT J AU Yin, WJ Wei, SH Yan, Y AF Yin, Wan-Jian Wei, Su-Huai Yan, Yanfa TI Control of one-dimensional magnetism in graphene via spontaneous hydrogenation of the grain boundary SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; BASIS-SET; CARBON AB We propose that control of one-dimensional (1D) magnetism in graphene could be made easier by spontaneous hydrogenation of chemically reactive grain boundaries (GBs) in polycrystalline graphenes. Unlike pristine graphene, where hydrogen adsorption favors the formation of zero-dimensional (0D) clusters, the defect cores (pentagon, heptagon and octagon) at the GBs in polycrystalline graphene promote hydrogenation along the GBs. The hydrogenation in polycrystalline graphene starts at the GBs, proceeds gradually towards the grain interior (GI) and results in smooth 1D graphane-graphene interfaces. Our calculations show that the type (ferro- or antiferro-magnetism) and strength of the magnetism can be controlled by controlling the orientation of GBs. Since GBs in single-layer graphenes can be fabricated in a controllable way in experiments, the hydrogenation of GBs could be a unique method to realize large-area magnetic graphenes for future spintronic applications. C1 [Yin, Wan-Jian; Yan, Yanfa] Univ Toledo, Dept Phys & Astron, Toledo, OH 43606 USA. [Wei, Su-Huai] Natl Renewable Energy Lab, Golden, CO USA. RP Yin, WJ (reprint author), Univ Toledo, Dept Phys & Astron, Toledo, OH 43606 USA. EM wanjian.yin@utoledo.edu; suhuai.wei@nrel.gov; yanfa.yan@utoledo.edu RI Yin, Wanjian/F-6738-2013 NR 38 TC 3 Z9 3 U1 2 U2 47 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PY 2013 VL 15 IS 21 BP 8271 EP 8275 DI 10.1039/c3cp50781e PG 5 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 139EV UT WOS:000318565500037 PM 23612720 ER PT J AU El Gabaly, F McCarty, KF Bluhm, H McDaniel, AH AF El Gabaly, Farid McCarty, Kevin F. Bluhm, Hendrik McDaniel, Anthony H. TI Oxidation stages of Ni electrodes in solid oxide fuel cell environments SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID NICKEL METAL; PHOTOELECTRON-SPECTROSCOPY; AMBIENT-PRESSURE; OXYGEN EVOLUTION; OXIDIZED NICKEL; WATER; SURFACE; FILMS; BEHAVIOR; GROWTH AB Nickel is the most commonly used anode for solid-oxide fuel cells (SOFC) due to its fast kinetics and low price. A leading cause of degradation in Ni electrodes is oxidation. Here we use operando ambient-pressure X-ray photoelectron spectroscopy (XPS) to chemically characterize the Ni electrode of a fuel cell anode during oxidation in a H-2/H2O atmosphere. We find three different stages of Ni oxidation in the model SOFC. In the first two stages, the Ni exposed to the gas remains metallic but the Ni at the interface with the zirconia electrolyte is oxidized. In the third oxidation stage, we find that Ni transforms to NiOOH, a phase not previously considered in the SOFC literature. We show that the transformation between Ni and NiOOH is reversible and is initiated at the Ni/gas interface. In addition we find that NiOOH stores charge, as evidenced by the stable discharge plateau (voltage) measured as this oxyhydroxide phase reduces to metallic Ni. C1 [El Gabaly, Farid; McCarty, Kevin F.; McDaniel, Anthony H.] Sandia Natl Labs, Livermore, CA 94551 USA. [Bluhm, Hendrik] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP El Gabaly, F (reprint author), Sandia Natl Labs, Livermore, CA 94551 USA. EM felgaba@sandia.gov RI McCarty, Kevin/F-9368-2012 OI McCarty, Kevin/0000-0002-8601-079X FU Office of Basic Energy Sciences, Division of Materials Sciences and Engineering of the U.S. Department of Energy; Sandia Laboratory Directed Research and Development program [DE-AC04-94AL85000]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This research was supported by the Office of Basic Energy Sciences, Division of Materials Sciences and Engineering of the U.S. Department of Energy and the Sandia Laboratory Directed Research and Development program under Contract DE-AC04-94AL85000. The Advanced Light Source and Beamline 11.0.2 are supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 36 TC 13 Z9 13 U1 1 U2 48 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PY 2013 VL 15 IS 21 BP 8334 EP 8341 DI 10.1039/c3cp50366f PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 139EV UT WOS:000318565500044 PM 23615670 ER PT J AU Thakur, P Conca, JL Dodge, CJ Francis, AJ Choppin, GR AF Thakur, P. Conca, J. L. Dodge, C. J. Francis, A. J. Choppin, G. R. TI Complexation thermodynamics and structural studies of trivalent actinide and lanthanide complexes with DTPA, MS-325 and HMDTPA SO RADIOCHIMICA ACTA LA English DT Article DE DTPA; HMDTPA; MS-325; Lanthanides; Actinides ID DIETHYLENETRIAMINEPENTAACETIC ACID; DIETHYLENETRIAMINE-N,N,N',N'',N''-PENTAACETIC ACID; CRYSTAL-STRUCTURES; HYDRATION NUMBER; DERIVATIVES; LUMINESCENCE; STABILITIES; EUROPIUM; SPECTRA; LIGANDS AB The protonation constants of DTPA (diethylenetriaminepentaacetic acid) and two derivatives of DTPA, 1-R(4,4-diphenyl cyclohexyl-phosphonyl-methyl diethylenentriamine-pentaacetic acid (MS-325) and (R)-hydroxymethyl-diethylenen-triaminepentaacetic acid (HMDTPA) were determined by potentiometric titration in 0.1 M NaClO4. The formation of 1: 1 complexes of Am3+, Cm3+ and Ln(3+) cations with these three ligands were investigated by potentiometric titration with competition by ethylenediaminetetraacetic acid (EDTA) and the solvent extraction method in aqueous solutions of I = 0.10 M NaClO4. The thermodynamic data of complexation were determined by the temperature dependence of the stability constants and by calorimetry. The complexation is exothermic and becomes weaker with increase in temperature. The complexation strength of these ligands follows the order: DTPA approximate to HMDTPA > MS-325. Eu3+/Cm3+ luminescence, EXAFS (Extended X-ray Absorption Fine Structure) and DFT (Density Functional Theory) calculations suggest that all three ligands are octadentate in the complex. In the complex, M(L)(2-) (L = DTPA, MS-325 and HMDTPA). The M3+ binds via five carboxylates oxygen atoms, three nitrogen atoms, and the complex contains one water of hydration. C1 [Thakur, P.; Choppin, G. R.] Florida State Univ, Dept Chem & Biochem, Tallahassee, FL 32306 USA. [Dodge, C. J.; Francis, A. J.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Francis, A. J.] Pohang Univ Sci & Technol, Div Adv Nucl Engn, Pohang, South Korea. RP Thakur, P (reprint author), Carlsbad Environm Monitoring & Res Ctr, 1400 Univ Dr, Carlsbad, NM 88220 USA. EM pthakur@cemrc.org FU USDOE-Office of Basic Sciences; World Class University (WCU) program through the National Research Foundation of Korea; Ministry of Education, Science and Technology [R31 - 30005] FX This research was supported by an USDOE-Office of Basic Sciences Contract and in part (AJF) by the World Class University (WCU) program through the National Research Foundation of Korea funded by the Ministry of Education, Science and Technology (R31 - 30005). We gratefully acknowledge the help of Dr. Bert Van De Burgt Department of Chemistry & Biochemistry Florida State University in data accumulations. Our thanks to the anonymous reviewer for thoughtful and constructive comments. NR 49 TC 5 Z9 5 U1 8 U2 36 PU OLDENBOURG VERLAG PI MUNICH PA LEKTORAT MINT, POSTFACH 80 13 60, D-81613 MUNICH, GERMANY SN 0033-8230 J9 RADIOCHIM ACTA JI Radiochim. Acta PY 2013 VL 101 IS 4 BP 221 EP 232 DI 10.1524/ract.2013.2018 PG 12 WC Chemistry, Inorganic & Nuclear; Nuclear Science & Technology SC Chemistry; Nuclear Science & Technology GA 140PZ UT WOS:000318668700003 ER PT J AU Mincher, BJ Precek, M Mezyk, SP Elias, G Martin, LR Paulenova, A AF Mincher, B. J. Precek, M. Mezyk, S. P. Elias, G. Martin, L. R. Paulenova, A. TI The redox chemistry of neptunium in gamma-irradiated aqueous nitric acid SO RADIOCHIMICA ACTA LA English DT Article DE Neptunium; Radiation chemistry; Nitrous acid; Redox chemistry ID PULSE-RADIOLYSIS; CATALYZED OXIDATION; HYDROGEN-ATOMS; RATE CONSTANTS; NITROUS-ACID; KINETICS; REACTIVITY; ELECTRON; NITRATE; SYSTEM AB The redox chemistry of neptunium in irradiated 4 M nitric acid was investigated using gamma-ray irradiation and UV/Vis spectroscopic measurements. Irradiation caused changes in the abundances of Np(V) and Np(VI) regardless of the initial fractional components of these oxidation states. At low absorbed doses Np(V) was oxidized to Np(VI) in irradiated solution, due to its reaction with oxidizing, radiolytically-produced, free radicals. However, when sufficient radiolytically-produced nitrous acid accumulated, the reduction of Np(VI) to Np(V) occurred, even at this high nitric acid concentration. Neptunium(IV) was not produced. A kinetic model which incorporates the standard water radiolysis reactions, estimated radical yields for 4 M HNO3, and rate constants for neptunium reactions available from the literature was used to successfully reproduce the experimental results. C1 [Mincher, B. J.; Elias, G.; Martin, L. R.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. [Precek, M.; Paulenova, A.] Oregon State Univ, Corvallis, OR 97331 USA. [Mezyk, S. P.] Calif State Univ Long Beach, Long Beach, CA 90820 USA. RP Mincher, BJ (reprint author), Idaho Natl Lab, POB 1625, Idaho Falls, ID 83415 USA. EM Bruce.Mincher@inl.gov RI Precek, Martin/G-5648-2014; Martin, Leigh/P-3167-2016; Mincher, Bruce/C-7758-2017 OI Precek, Martin/0000-0002-5790-5543; Martin, Leigh/0000-0001-7241-7110; FU INL Laboratory Directed Research and Development (LDRD) program under DOE Idaho Operations Office [DE-AC07-05ID14517] FX This work was supported through the INL Laboratory Directed Research and Development (LDRD) program, under DOE Idaho Operations Office Contract DE-AC07-05ID14517. NR 33 TC 6 Z9 6 U1 0 U2 25 PU OLDENBOURG VERLAG PI MUNICH PA LEKTORAT MINT, POSTFACH 80 13 60, D-81613 MUNICH, GERMANY SN 0033-8230 J9 RADIOCHIM ACTA JI Radiochim. Acta PY 2013 VL 101 IS 4 BP 259 EP 265 DI 10.1524/ract.2013.2013 PG 7 WC Chemistry, Inorganic & Nuclear; Nuclear Science & Technology SC Chemistry; Nuclear Science & Technology GA 140PZ UT WOS:000318668700007 ER PT J AU Holliday, K Dardenne, K Walther, C Stumpf, T AF Holliday, K. Dardenne, K. Walther, C. Stumpf, T. TI The incorporation of europium into apatite: a new explanation SO RADIOCHIMICA ACTA LA English DT Article DE Apatite; Europium; TRLFS; EXAFS; Incorporation; Mechanism ID SPECTROSCOPY; CHEMISTRY; IONS; LUMINESCENCE; IFEFFIT; OLIVINE; SYSTEM; MODEL AB Time resolved laser fluorescence spectroscopy (TRLFS) and X-ray absorption fine structure (XAFS) are used as complimentary techniques to show that the heterovalent incorporation of europium into apatite at temperatures relevant to environmental and biological processes occurs at grain boundaries and not the crystallographic calcium sites as previously presumed. For this study, we focus on mechanisms at the solid solution interface and therefore define this temperature regime as the range in which liquid water exists (0-100 degrees C). Site-selective TRLFS show that the local Eu3+ symmetry does not match the presumed crystallographic site of incorporation. This is confirmed by XAFS results that show a deviation from the local environment in apatite. The transition of this amorphous europium to a crystallographic calcium site upon heating is then explained by grain growth and followed through a transition species by TRLFS. C1 [Holliday, K.; Dardenne, K.; Walther, C.; Stumpf, T.] Karlsruhe Inst Technol, Inst Nukl Entsorgung, D-76021 Karlsruhe, Germany. [Holliday, K.] Lawrence Livermore Natl Lab, Div Mat, Livermore, CA USA. [Walther, C.] Leibniz Univ Hannover, Inst Radiookol & Strahlenschutz, D-30419 Hannover, Germany. RP Holliday, K (reprint author), Karlsruhe Inst Technol, Inst Nukl Entsorgung, POB 3640, D-76021 Karlsruhe, Germany. EM holliday7@llnl.gov RI Dardenne, Kathy/A-2519-2017 OI Dardenne, Kathy/0000-0003-1286-1855 FU Helmholtz Gemeinshaft Deutscher Forschungszentren (HGF); LLNL [DE-AC52-07NA27344] FX We would like to thank Sebastian Buchner for technical assistance with TRLFS measurements. This work was cofinanced by the Helmholtz Gemeinshaft Deutscher Forschungszentren (HGF) by supporting the Helmholtz-Hochschul-Nachwuchsgruppe "Aufklarung geochemischer Reaktionsmechanismen an der Wasser/Mineralphasen Grenzflache". We thank the ANKA synchrotron source for providing the beamtime. Prepared by LLNL under Contract DE-AC52-07NA27344. NR 38 TC 2 Z9 2 U1 1 U2 22 PU WALTER DE GRUYTER GMBH PI BERLIN PA GENTHINER STRASSE 13, D-10785 BERLIN, GERMANY SN 0033-8230 J9 RADIOCHIM ACTA JI Radiochim. Acta PY 2013 VL 101 IS 4 BP 267 EP 272 DI 10.1524/ract.2013.2023 PG 6 WC Chemistry, Inorganic & Nuclear; Nuclear Science & Technology SC Chemistry; Nuclear Science & Technology GA 140PZ UT WOS:000318668700008 ER PT J AU Conway, JM Konrad, BP Coombs, D AF Conway, Jessica M. Konrad, Bernhard P. Coombs, Daniel TI STOCHASTIC ANALYSIS OF PRE- AND POSTEXPOSURE PROPHYLAXIS AGAINST HIV INFECTION SO SIAM JOURNAL ON APPLIED MATHEMATICS LA English DT Article DE HIV; viral dynamics; branching process; preexposure prophylaxis; postexposure prophylaxis; HIV prevention ID HUMAN-IMMUNODEFICIENCY-VIRUS; HEPATITIS-C VIRUS; PREEXPOSURE PROPHYLAXIS; VIRAL LOAD; IN-VIVO; ANTIRETROVIRAL THERAPY; MUCOSAL TRANSMISSION; POPULATION-DYNAMICS; COITAL ACT; PREVENTION AB The events that occur following HIV exposure, preceding any detectable infection, are difficult to study experimentally. However, there is considerable evidence that these events can be influenced by the action of antiretroviral drugs, taken either as pre-or postexposure prophylaxis (PrEP and PEP, respectively). We present simple theoretical models of HIV dynamics immediately following exposure, and apply these models to understanding how drug prophylaxis can act to reduce the risk of infection. Because HIV infection following exposure is a relatively rare event, we work with stochastic models which we base on continuous-time branching processes, allowing us to compute the risk of infection under different scenarios. We obtain analytical solutions for viral extinction probabilities, allowing us to avoid extensive computer simulations. We predict in the case of PrEP that reverse transcriptase inhibitors should be somewhat more effective than protease inhibitors and also that single drugs should be nearly as effective as a combination approach. We then model viral dynamics under PEP and find that fast initiation of therapy is essential for risk reduction. However, we predict that a two-week PEP regimen would be nearly as effective as the current recommendation of four weeks of therapy. Our work provides a coherent platform for studying the early dynamics of HIV and indicates possible directions for experimental and theoretical work. C1 [Conway, Jessica M.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Konrad, Bernhard P.; Coombs, Daniel] Univ British Columbia, Dept Math, Vancouver, BC V6T 1Z2, Canada. [Konrad, Bernhard P.; Coombs, Daniel] Univ British Columbia, Inst Appl Math, Vancouver, BC V6T 1Z2, Canada. RP Conway, JM (reprint author), Los Alamos Natl Lab, T-6, Los Alamos, NM 87545 USA. EM conway@lanl.gov; konradbe@math.ubc.ca; coombs@math.ubc.ca OI Coombs, Daniel/0000-0002-8038-6278 FU Natural Science and Engineering Research Council of Canada; Canadian Institutes of Health Research [HFE-105370, HET 85520]; Pacific Institute for Mathematical Sciences through the International Graduate Training Centre in Mathematical Biology FX This work was supported by the Natural Science and Engineering Research Council of Canada and by the Canadian Institutes of Health Research [funding reference number HFE-105370 to JMC; grant HET 85520], the Pacific Institute for Mathematical Sciences through the International Graduate Training Centre in Mathematical Biology, and was enabled by the use of computing resources provided by WestGrid and Compute/Calcul Canada. NR 53 TC 6 Z9 6 U1 0 U2 8 PU SIAM PUBLICATIONS PI PHILADELPHIA PA 3600 UNIV CITY SCIENCE CENTER, PHILADELPHIA, PA 19104-2688 USA SN 0036-1399 J9 SIAM J APPL MATH JI SIAM J. Appl. Math. PY 2013 VL 73 IS 2 BP 904 EP 928 DI 10.1137/120876800 PG 25 WC Mathematics, Applied SC Mathematics GA 136IO UT WOS:000318355800014 ER PT J AU Chen, J AF Chen, Jie TI ON THE USE OF DISCRETE LAPLACE OPERATOR FOR PRECONDITIONING KERNEL MATRICES SO SIAM JOURNAL ON SCIENTIFIC COMPUTING LA English DT Article DE Laplace operator; preconditioning; kernel matrix; Toeplitz matrix; stiffness matrix ID SEQUENCES; SYSTEMS AB This paper presents a preconditioning strategy applied to certain types of kernel matrices that are increasingly ill-conditioned. The ill-conditioning of these matrices is tied to the unbounded variation of the Fourier transform of the kernel function. Hence, the basic idea is to differentiate the kernel in order to suppress the variation. The idea resembles some existing preconditioning methods for Toeplitz matrices, where the theory heavily relies on the underlying fixed generating function. The theory does not apply to the case of a fixed domain with increasingly fine discretizations because the generating function depends on the grid size. For this case, we prove equal distribution results on the spectrum of the resulting matrices. Furthermore, the proposed preconditioning technique also applies to non-Toeplitz matrices, thus eliminating the reliance on a regular grid structure of the points. The preconditioning strategy can be used to accelerate an iterative solver for solving linear systems with respect to kernel matrices. C1 Argonne Natl Lab, Div Math & Comp Sci, Argonne, IL 60439 USA. RP Chen, J (reprint author), Argonne Natl Lab, Div Math & Comp Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM jiechen@mcs.anl.gov FU U.S. Department of Energy [DE-AC02-06CH11357]; UChicago Argonne, LLC, Operator of Argonne National Laboratory ("Argonne") [DE-AC02-06CH11357]; U.S. Department of Energy FX This work was supported by the U.S. Department of Energy under contract DE-AC02-06CH11357. This work was performed by UChicago Argonne, LLC, Operator of Argonne National Laboratory ("Argonne") under contract DE-AC02-06CH11357 with the U.S. Department of Energy. The U.S. government retains for itself, and others acting on its behalf, a paid-up, nonexclusive, irrevocable worldwide license in said article to reproduce, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, by or on behalf of the government. NR 22 TC 1 Z9 1 U1 0 U2 2 PU SIAM PUBLICATIONS PI PHILADELPHIA PA 3600 UNIV CITY SCIENCE CENTER, PHILADELPHIA, PA 19104-2688 USA SN 1064-8275 EI 1095-7197 J9 SIAM J SCI COMPUT JI SIAM J. Sci. Comput. PY 2013 VL 35 IS 2 BP A577 EP A602 DI 10.1137/120874527 PG 26 WC Mathematics, Applied SC Mathematics GA 136ZT UT WOS:000318404100003 ER PT J AU Lipnikov, K Svyatskiy, D Vassilevski, Y AF Lipnikov, K. Svyatskiy, D. Vassilevski, Y. TI ANDERSON ACCELERATION FOR NONLINEAR FINITE VOLUME SCHEME FOR ADVECTION-DIFFUSION PROBLEMS SO SIAM JOURNAL ON SCIENTIFIC COMPUTING LA English DT Article DE advection-diffusion equation; finite volume method; discrete maximum principle; positivity preservation; Picard's method; Anderson acceleration ID POLYGONAL MESHES; MAXIMUM-PRINCIPLES; POLYHEDRAL MESHES; EQUATIONS; SYSTEMS; ROBUSTNESS AB We consider the solution of systems of nonlinear algebraic equations that appear in a positivity preserving finite volume scheme for steady-state advection-diffusion equations. We propose and analyze numerically an efficient strategy for accelerating the Picard method when it is applied to these systems. The strategy is based on the Anderson acceleration and the adaptive inexact solution of linear systems. We demonstrate its numerical robustness for three black-box preconditioners. C1 [Lipnikov, K.; Svyatskiy, D.] Los Alamos Natl Lab, Div Theoret, Appl Math & Plasma Phys Grp, Los Alamos, NM 87545 USA. [Vassilevski, Y.] Russian Acad Sci, Inst Numer Math, Moscow 119333, Russia. RP Lipnikov, K (reprint author), Los Alamos Natl Lab, Div Theoret, Appl Math & Plasma Phys Grp, Los Alamos, NM 87545 USA. EM lipnikov@lanl.gov; dasvyat@lanl.gov; vasilevs@dodo.inm.ras.ru RI Vassilevski, Yuri/A-6068-2016 FU National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396]; DOE Office of Science Advanced Scientific Computing Research (ASCR) Program in Applied Mathematics Research FX Submitted to the journal's Methods and Algorithms for Scientific Computing section February 28, 2012; accepted for publication (in revised form) December 7, 2012; published electronically April 23, 2013. This work was carried out under the auspices of the National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory under Contract DE-AC52-06NA25396 and the DOE Office of Science Advanced Scientific Computing Research (ASCR) Program in Applied Mathematics Research.; This work was carried out under the auspices of the National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory under Contract DE-AC52-06NA25396 and the DOE Office of Science Advanced Scientific Computing Research (ASCR) Program in Applied Mathematics. NR 40 TC 4 Z9 4 U1 0 U2 3 PU SIAM PUBLICATIONS PI PHILADELPHIA PA 3600 UNIV CITY SCIENCE CENTER, PHILADELPHIA, PA 19104-2688 USA SN 1064-8275 EI 1095-7197 J9 SIAM J SCI COMPUT JI SIAM J. Sci. Comput. PY 2013 VL 35 IS 2 BP A1120 EP A1136 DI 10.1137/120867846 PG 17 WC Mathematics, Applied SC Mathematics GA 136ZT UT WOS:000318404100026 ER PT J AU Vecharynski, E Knyazev, AV AF Vecharynski, Eugene Knyazev, Andrew V. TI ABSOLUTE VALUE PRECONDITIONING FOR SYMMETRIC INDEFINITE LINEAR SYSTEMS SO SIAM JOURNAL ON SCIENTIFIC COMPUTING LA English DT Article DE preconditioning; linear system; preconditioned minimal residual method; polar decomposition; matrix absolute value; multigrid; polynomial filtering ID STABILIZED STOKES SYSTEMS; CONJUGATE-GRADIENT METHOD; FAST ITERATIVE SOLUTION; HELMHOLTZ-EQUATION; SHIFTED-LAPLACIAN; GMRES; ALGORITHM AB We introduce a novel strategy for constructing symmetric positive definite (SPD) preconditioners for linear systems with symmetric indefinite matrices. The strategy, called absolute value preconditioning, is motivated by the observation that the preconditioned minimal residual method with the inverse of the absolute value of the matrix as a preconditioner converges to the exact solution of the system in at most two steps. Neither the exact absolute value of the matrix nor its exact inverse are computationally feasible to construct in general. However, we provide a practical example of an SPD preconditioner that is based on the suggested approach. In this example we consider a model problem with a shifted discrete negative Laplacian and suggest a geometric multigrid (MG) preconditioner, where the inverse of the matrix absolute value appears only on the coarse grid, while operations on finer grids are based on the Laplacian. Our numerical tests demonstrate practical effectiveness of the new MG preconditioner, which leads to a robust iterative scheme with minimalist memory requirements. C1 [Vecharynski, Eugene] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, Berkeley, CA 94720 USA. [Knyazev, Andrew V.] Univ Colorado, Dept Math & Stat Sci, Denver, CO 80217 USA. [Knyazev, Andrew V.] Mitsubishi Elect Res Labs, Cambridge, MA 02139 USA. RP Vecharynski, E (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, Berkeley, CA 94720 USA. EM eugene.vecharynski@gmail.com; andrew.knyazev@ucdenver.edu RI Knyazev, Andrew/H-2274-2011 OI Knyazev, Andrew/0000-0002-1635-3711 FU National Science Foundation [1115734] FX This work is partially supported by National Science Foundation grant 1115734. NR 45 TC 5 Z9 5 U1 3 U2 7 PU SIAM PUBLICATIONS PI PHILADELPHIA PA 3600 UNIV CITY SCIENCE CENTER, PHILADELPHIA, PA 19104-2688 USA SN 1064-8275 EI 1095-7197 J9 SIAM J SCI COMPUT JI SIAM J. Sci. Comput. PY 2013 VL 35 IS 2 BP A696 EP A718 DI 10.1137/120886686 PG 23 WC Mathematics, Applied SC Mathematics GA 136ZT UT WOS:000318404100008 ER PT J AU Brown, J Smith, B Ahmadia, A AF Brown, Jed Smith, Barry Ahmadia, Aron TI ACHIEVING TEXTBOOK MULTIGRID EFFICIENCY FOR HYDROSTATIC ICE SHEET FLOW SO SIAM JOURNAL ON SCIENTIFIC COMPUTING LA English DT Article DE hydrostatic; ice sheet; Newton-Krylov; multigrid; preconditioning ID HIGHER-ORDER; MODEL; GLACIOLOGY; PRECONDITIONER; APPROXIMATION; VELOCITY; STREAMS AB The hydrostatic equations for ice sheet flow offer improved fidelity compared with the shallow ice approximation and shallow stream approximation popular in today's ice sheet models. Nevertheless, they present a serious bottleneck because they require the solution of a three-dimensional (3D) nonlinear system, as opposed to the two-dimensional system present in the shallow stream approximation. This 3D system is posed on high-aspect domains with strong anisotropy and variation in coefficients, making it expensive to solve with current methods. This paper presents a Newton-Krylov multigrid solver for the hydrostatic equations that demonstrates textbook multigrid efficiency (an order of magnitude reduction in residual per iteration and solution of the fine-level system at a small multiple of the cost of a residual evaluation). Scalability on Blue Gene/P is demonstrated, and the method is compared to various algebraic methods that are in use or have been proposed as viable approaches. C1 [Brown, Jed; Smith, Barry] Argonne Natl Lab, Div Math & Comp Sci, Argonne, IL 60439 USA. [Ahmadia, Aron] King Abdullah Univ Sci & Technol, Supercomp Lab, Thuwal 293556900, Makkah, Saudi Arabia. RP Brown, J (reprint author), Argonne Natl Lab, Div Math & Comp Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM jedbrown@mcs.anl.gov; bsmith@mcs.anl.gov; aron.ahmadia@kaust.edu.sa OI Smith, Barry/0000-0001-5955-8111 FU Swiss National Science Foundation Grant [200021-113503/1]; U.S. Department of Energy's Office of Science Ice Sheet Initiative for CL-imate ExtremeS program [DE-AC02-06CH11357]; Shaheen Supercomputing Laboratory at KAUST; U.S. Department of Energy Office of Science laboratory [DE-AC02-06CH11357] FX Submitted to the journal's Computational Methods in Science and Engineering section May 18, 2011; accepted for publication (in revised form) July 2, 2012; published electronically March 12, 2013. This work was supported by Swiss National Science Foundation Grant 200021-113503/1, U.S. Department of Energy's Office of Science Ice Sheet Initiative for CL-imate ExtremeS program under Contract DE-AC02-06CH11357, and the Shaheen Supercomputing Laboratory at KAUST. This manuscript was created by UChicago Argonne, LLC, Operator of Argonne National Laboratory ("Argonne"). Argonne, a U.S. Department of Energy Office of Science laboratory, is operated under contract DE-AC02-06CH11357. The U.S. Government retains for itself, and others acting on its behalf, a paid-up nonexclusive, irrevocable worldwide license in said article to reproduce, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, by or on behalf of the government. NR 38 TC 13 Z9 13 U1 0 U2 9 PU SIAM PUBLICATIONS PI PHILADELPHIA PA 3600 UNIV CITY SCIENCE CENTER, PHILADELPHIA, PA 19104-2688 USA SN 1064-8275 EI 1095-7197 J9 SIAM J SCI COMPUT JI SIAM J. Sci. Comput. PY 2013 VL 35 IS 2 BP B359 EP B375 DI 10.1137/110834512 PG 17 WC Mathematics, Applied SC Mathematics GA 136ZT UT WOS:000318404100033 ER PT J AU Owhadi, H Scovel, C Sullivan, TJ McKerns, M Ortiz, M AF Owhadi, H. Scovel, C. Sullivan, T. J. McKerns, M. Ortiz, M. TI Optimal Uncertainty Quantification SO SIAM REVIEW LA English DT Article DE uncertainty quantification; concentration inequalities; sensitivity analysis; Markov-Krein-type reduction theorems for generalized Chebyshev optimization problems ID BOUNDED RANDOM-VARIABLES; EXTREME-POINTS; TERMINAL BALLISTICS; INEQUALITIES; SUMS; DISTRIBUTIONS; OPTIMIZATION; CONVERGENCE; CONSISTENCY; STATISTICS AB We propose a rigorous framework for uncertainty quantification (UQ) in which the UQ objectives and its assumptions/information set are brought to the forefront. This framework, which we call optimal uncertainty quantification (OUQ), is based on the observation that, given a set of assumptions and information about the problem, there exist optimal bounds on uncertainties: these are obtained as values of well-defined optimization problems corresponding to extremizing probabilities of failure, or of deviations, subject to the constraints imposed by the scenarios compatible with the assumptions and information. In particular, this framework does not implicitly impose inappropriate assumptions, nor does it repudiate relevant information. Although OUQ optimization problems are extremely large, we show that under general conditions they have finite-dimensional reductions. As an application, we develop optimal concentration inequalities (OCI) of Hoeffding and McDiarmid type. Surprisingly, these results show that uncertainties in input parameters, which propagate to output uncertainties in the classical sensitivity analysis paradigm, may fail to do so if the transfer functions (or probability distributions) are imperfectly known. We show how, for hierarchical structures, this phenomenon may lead to the nonpropagation of uncertainties or information across scales. In addition, a general algorithmic framework is developed for OUQ and is tested on the Caltech surrogate model for hypervelocity impact and on the seismic safety assessment of truss structures, suggesting the feasibility of the framework for important complex systems. The introduction of this paper provides both an overview of the paper and a self-contained minitutorial on the basic concepts and issues of UQ. C1 [Owhadi, H.; Sullivan, T. J.] CALTECH, Pasadena, CA 91125 USA. [Scovel, C.] Los Alamos Natl Lab, Los Alamos, NM USA. [McKerns, M.] CALTECH, Ctr Adv Comp Res, Pasadena, CA 91125 USA. [Ortiz, M.] CALTECH, Grad Aeronaut Labs, Dept Aeronaut, Pasadena, CA 91125 USA. RP Owhadi, H (reprint author), CALTECH, Pasadena, CA 91125 USA. EM owhadi@caltech.edu; jcs@lanl.gov; tjs@caltech.edu; mmckerns@caltech.edu; ortiz@aero.caltech.edu FU Department of Energy National Nuclear Security Administration through Caltech's ASC/PSAAP Center for the Predictive Modeling and Simulation of High Energy Density Dynamic Response of Materials [DE-FC52-08NA28613] FX Received by the editors September 7, 2010; accepted for publication (in revised form) May 22, 2012; published electronically May 8, 2013. This work was partially supported by the Department of Energy National Nuclear Security Administration under award DE-FC52-08NA28613 through Caltech's ASC/PSAAP Center for the Predictive Modeling and Simulation of High Energy Density Dynamic Response of Materials. NR 101 TC 19 Z9 19 U1 1 U2 21 PU SIAM PUBLICATIONS PI PHILADELPHIA PA 3600 UNIV CITY SCIENCE CENTER, PHILADELPHIA, PA 19104-2688 USA SN 0036-1445 EI 1095-7200 J9 SIAM REV JI SIAM Rev. PY 2013 VL 55 IS 2 BP 271 EP 345 DI 10.1137/10080782X PG 75 WC Mathematics, Applied SC Mathematics GA 142GS UT WOS:000318785900002 ER PT J AU Wild, SM Shoemaker, CA AF Wild, Stefan M. Shoemaker, Christine A. TI Global Convergence of Radial Basis Function Trust-Region Algorithms for Derivative-Free Optimization SO SIAM REVIEW LA English DT Article DE derivative-free optimization; radial basis functions; trust-region methods; nonlinear optimization ID PARALLEL PATTERN SEARCH; NONLINEAR OPTIMIZATION; UNCONSTRAINED OPTIMIZATION; GEOMETRY AB We analyze globally convergent, derivative-free trust-region algorithms relying on radial basis function interpolation models. Our results extend the recent work of Conn, Scheinberg, and Vicente [SIAM J. Optim., 20 (2009), pp. 387-415] to fully linear models that have a nonlinear term. We characterize the types of radial basis functions that fit in our analysis and thus show global convergence to first-order critical points for the ORBIT algorithm of Wild, Regis, and Shoemaker [SIAM J. Sci. Comput., 30 (2008), pp. 3197-3219]. Using ORBIT, we present numerical results for different types of radial basis functions on a series of test problems. We also demonstrate the use of ORBIT in finding local minima on a computationally expensive environmental engineering problem involving remediation of contaminated groundwater. C1 [Wild, Stefan M.] Argonne Natl Lab, Div Math & Comp Sci, Argonne, IL 60439 USA. [Shoemaker, Christine A.] Cornell Univ, Sch Civil & Environm Engn, Ithaca, NY 14853 USA. [Shoemaker, Christine A.] Cornell Univ, Sch Operat Res & Informat Engn, Ithaca, NY 14853 USA. RP Wild, SM (reprint author), Argonne Natl Lab, Div Math & Comp Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM wild@mcs.anl.gov; cas12@cornell.edu RI Wild, Stefan/P-4907-2016 OI Wild, Stefan/0000-0002-6099-2772 FU Argonne, a U.S. Department of Energy (DOE) Office of Science laboratory [DE-AC02-06CH11357]; DOE Computational Science Graduate Fellowship [DE-FG02-97ER25308]; Applied Mathematics activity within the DOE Office of Science's Advanced Scientific Computing Research program; NSF [BES-022917, CBET-0756575, CCF-0305583, DMS-0434390] FX Mathematics and Computer Science Division, Argonne National Laboratory, Argonne, IL 60439 (wild@mcs.anl.gov). Argonne, a U.S. Department of Energy (DOE) Office of Science laboratory, is operated under contract DE-AC02-06CH11357. The work of this author was supported by a DOE Computational Science Graduate Fellowship under grant DE-FG02-97ER25308 and by the Applied Mathematics activity within the DOE Office of Science's Advanced Scientific Computing Research program.; School of Civil and Environmental Engineering and School of Operations Research and Information Engineering, Cornell University, Hollister Hall, Ithaca, NY 14853 (cas12@cornell.edu). The work of this author was supported by NSF grants BES-022917, CBET-0756575, CCF-0305583, and DMS-0434390. NR 40 TC 15 Z9 15 U1 0 U2 11 PU SIAM PUBLICATIONS PI PHILADELPHIA PA 3600 UNIV CITY SCIENCE CENTER, PHILADELPHIA, PA 19104-2688 USA SN 0036-1445 EI 1095-7200 J9 SIAM REV JI SIAM Rev. PY 2013 VL 55 IS 2 BP 349 EP 371 DI 10.1137/120902434 PG 23 WC Mathematics, Applied SC Mathematics GA 142GS UT WOS:000318785900003 ER PT J AU Yang, L Zhu, ZH Yu, XY Thevuthasan, S Cowin, JP AF Yang, Li Zhu, Zihua Yu, Xiao-Ying Thevuthasan, Suntharampillai Cowin, James P. TI Performance of a microfluidic device for in situ ToF-SIMS analysis of selected organic molecules at aqueous surfaces SO ANALYTICAL METHODS LA English DT Article ID ION MASS-SPECTROMETRY; X-RAY SPECTROSCOPY; LIQUID WATER; AIR/WATER INTERFACE; MICROJETS; DYNAMICS; EVAPORATION; FILMS; BEAM AB In this study, we report new results concerning the analytical performance of a novel portable vacuum compatible device enabling in situ study of aqueous surfaces using vacuum-based surface analysis tools. The surfaces of aqueous solutions of three representative organic molecules (formic acid, glycerol, and glutamic acid) were analyzed using time-of-flight secondary ion mass spectrometry (ToF-SIMS). Their molecular signals were successfully observed. The device can be operated without interruption in vacuum for up to 8 hours, and SIMS measurements are feasible at any time in this time range. The stability testing of our device under primary ion beam bombardment shows that high fluence (6 x 10(12) ions per cm(2) s(-1)) measurements can be operated continuously for up to 30 minutes without any significant damage to the aperture. However, extra-high fluence measurements (>1 x 10(14) ions per cm(2) s(-1)) may lead to rapid boiling in the aperture, and the aqueous solutions may spread out quickly. Device reproducibility is studied for both consecutive measurements over a short period of time (e.g., 5 min) and intermittent measurements over a long time (e. g., several hours). The relative standard deviation (RSD) for molecular ion signals was determined to be less than 15% for consecutive measurements in 5 min. As to total counts, the RSD is determined to be less than 1% for each chemical compound. Higher RSDs of +/- 40-50% were obtained for intermittent measurements in a few hours, both acceptable for semi-quantitative analysis. In addition, the detection limits of formic acid, glycerol, and glutamic acid are estimated to be 0.04%, 0.008%, and 0.002% (weight ratio), respectively. C1 [Yang, Li; Cowin, James P.] Pacific NW Natl Lab, Chem & Mat Sci Div, Richland, WA 99354 USA. [Yang, Li; Zhu, Zihua; Thevuthasan, Suntharampillai] Pacific NW Natl Lab, WR Wiley Environm Mol Sci Lab, Richland, WA 99354 USA. [Yu, Xiao-Ying] Pacific NW Natl Lab, Atmospher Sci & Global Climate Change Div, Richland, WA 99354 USA. RP Zhu, ZH (reprint author), Pacific NW Natl Lab, WR Wiley Environm Mol Sci Lab, Richland, WA 99354 USA. EM zihua.zhu@pnnl.gov; xiaoying.yu@pnnl.gov RI Zhu, Zihua/K-7652-2012; Yu, Xiao-Ying/L-9385-2013 OI Yu, Xiao-Ying/0000-0002-9861-3109 FU Department of Energy (DOE) Division of Chemical Sciences, Geosciences, and Biosciences (BES Chemical Sciences grant) [KC-0301020-16248]; Office of Biological and Environmental Research (OBER); Use at Facility Funds (UAFF) of the Pacific Northwest National Laboratory (PNNL); PNNL Chemical Imaging Initiative LDRD (Laboratory Directed Research and Development) Fund; OBER FX We are grateful for the support from the Department of Energy (DOE) Division of Chemical Sciences, Geosciences, and Biosciences (BES Chemical Sciences grant, KC-0301020-16248), the Office of Biological and Environmental Research (OBER), the Use at Facility Funds (UAFF) of the Pacific Northwest National Laboratory (PNNL), and the PNNL Chemical Imaging Initiative LDRD (Laboratory Directed Research and Development) Fund. The research was performed in the W. R. Wiley Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by OBER and located at PNNL. PNNL is operated for DOE by Battelle. A Battelle patent (Intellectual Property Report no. 16961-E) was filed based on this invention. NR 38 TC 11 Z9 11 U1 0 U2 34 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1759-9660 EI 1759-9679 J9 ANAL METHODS-UK JI Anal. Methods PY 2013 VL 5 IS 10 BP 2515 EP 2522 DI 10.1039/c3ay26513g PG 8 WC Chemistry, Analytical; Food Science & Technology; Spectroscopy SC Chemistry; Food Science & Technology; Spectroscopy GA 135US UT WOS:000318314700012 ER PT J AU Comolli, LR Siegerist, CE Shin, SH Bertozzi, C Regan, W Zettl, A De Yoreo, J AF Comolli, Luis R. Siegerist, Cristina E. Shin, Seong-Ho Bertozzi, Carolyn Regan, William Zettl, Alex De Yoreo, Jim TI Conformational Transitions at an S-Layer Growing Boundary Resolved by Cryo-TEM SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE conformational transitions; electron microscopy; nanostructures; oligomeric intermediates; self-assembly ID PROTEINS; TUBULIN; GROWTH C1 [Comolli, Luis R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. [Siegerist, Cristina E.] Http Www Cristinasiegerist Com ComputingVisualiza, Berkeley, CA 94708 USA. [Shin, Seong-Ho; De Yoreo, Jim] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Regan, William; Zettl, Alex] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Regan, William; Zettl, Alex] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Bertozzi, Carolyn] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. RP Comolli, LR (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. EM lrcomolli@lbl.gov RI Foundry, Molecular/G-9968-2014; Zettl, Alex/O-4925-2016; OI Zettl, Alex/0000-0001-6330-136X; Regan, William/0000-0003-0143-9827 FU Office of Science, Office of Basic Energy Sciences, Biological and Environmental Research, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was performed at Lawrence Berkeley National Laboratory, with support from the Office of Science, Office of Basic Energy Sciences, Biological and Environmental Research, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 24 TC 8 Z9 8 U1 1 U2 33 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PY 2013 VL 52 IS 18 BP 4829 EP 4832 DI 10.1002/anie.201300543 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA 132ZO UT WOS:000318107400015 PM 23564404 ER PT J AU Palaniappan, KK Ramirez, RM Bajaj, VS Wemmer, DE Pines, A Francis, MB AF Palaniappan, Krishnan K. Ramirez, R. Matthew Bajaj, Vikram S. Wemmer, David E. Pines, Alexander Francis, Matthew B. TI Molecular Imaging of Cancer Cells Using a Bacteriophage-Based 129Xe NMR Biosensor SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE cancer cells; NMR imaging; protein bioconjugation; viral capsids; xenon ID NUCLEAR-MAGNETIC-RESONANCE; LASER-POLARIZED XE-129; GROWTH-FACTOR RECEPTOR; HYPERPOLARIZED XE-129; FUNCTIONALIZED XENON; FILAMENTOUS PHAGE; CONTRAST AGENTS; PARACEST AGENTS; SPECTROSCOPY; CRYPTOPHANE C1 [Palaniappan, Krishnan K.; Ramirez, R. Matthew; Bajaj, Vikram S.; Wemmer, David E.; Pines, Alexander; Francis, Matthew B.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Ramirez, R. Matthew; Bajaj, Vikram S.; Pines, Alexander; Francis, Matthew B.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Wemmer, David E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Francis, MB (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM mbfrancis@berkeley.edu FU U.S. Department of Defense Cancer Research Program [BC016995]; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Science and Engineering [DE-AC02-05CH112] FX This work was supported by grants from the U.S. Department of Defense Cancer Research Program (grant number BC016995, M.B.F.) and by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Science and Engineering under contract number DE-AC02-05CH112 (A.P.). NR 54 TC 39 Z9 39 U1 3 U2 64 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PY 2013 VL 52 IS 18 BP 4849 EP 4853 DI 10.1002/anie.201300170 PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA 132ZO UT WOS:000318107400020 PM 23554263 ER PT J AU Kuvychko, IV Castro, KP Deng, SHM Wang, XB Strauss, SH Boltalina, OV AF Kuvychko, Igor V. Castro, Karlee P. Deng, S. H. M. Wang, Xue-Bin Strauss, Steven H. Boltalina, Olga V. TI Taming Hot CF3 Radicals: Incrementally Tuned Families of Polyarene Electron Acceptors for Air-Stable Molecular Optoelectronics SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE electrochemistry; electron affinity; polycyclic aromatic hydrocarbons; synthetic methods; trifluoromethylation ID ORGANIC SEMICONDUCTORS; AROMATIC-COMPOUNDS; PERFLUOROALKYLATION; TRIFLUOROMETHYLATION; AFFINITIES C1 [Kuvychko, Igor V.; Castro, Karlee P.; Strauss, Steven H.; Boltalina, Olga V.] Colorado State Univ, Dept Chem, Ft Collins, CO 80523 USA. [Deng, S. H. M.; Wang, Xue-Bin] Pacific NW Natl Lab, Chem & Mat Sci Div, Richland, WA 99352 USA. RP Kuvychko, IV (reprint author), Colorado State Univ, Dept Chem, Ft Collins, CO 80523 USA. EM igor.kuvychko@gmail.com; xuebin.wang@pnnl.gov; steven.strauss@colostate.edu; olga.boltalina@colostate.edu FU U.S. Department of Energy (DOE), Division of Chemical Sciences, Geosciences and Biosciences, Office of Basic Energy Sciences; DOE's Office of Biological and Environmental Research FX We thank the U.S. NSF (CHE-1012468 (SHS/OVB) and the Colorado State University Research Foundation for generous support. The PES work was supported by the U.S. Department of Energy (DOE), Division of Chemical Sciences, Geosciences and Biosciences, Office of Basic Energy Sciences and was performed at the EMSL, a national scientific user facility sponsored by DOE's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory, which is operated for DOE by Battelle. NR 28 TC 16 Z9 16 U1 2 U2 53 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PY 2013 VL 52 IS 18 BP 4871 EP 4874 DI 10.1002/anie.201300085 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA 132ZO UT WOS:000318107400025 PM 23526691 ER PT J AU Jacobson, AR Light, TEL Hamlin, T Nemzek, R AF Jacobson, A. R. Light, T. E. L. Hamlin, T. Nemzek, R. TI Joint radio and optical observations of the most radio-powerful intracloud lightning discharges SO ANNALES GEOPHYSICAE LA English DT Article DE Meteorology and atmospheric dynamics; Atmospheric electricity; Lightning ID TRANSIONOSPHERIC PULSE PAIRS; NARROW BIPOLAR EVENTS; ALAMOS SFERIC ARRAY; FORTE SATELLITE; PHOTODIODE DETECTOR; TRANSIENT DETECTOR; DETECTION NETWORK; VHF; FREQUENCY; EMISSIONS AB The most radio-powerful intracloud lightning emissions are associated with a phenomenon variously called "narrow bipolar events" or "compact intracloud discharges". This article examines in detail the coincidence and timing relationship between, on the one hand, the most radio-powerful intracloud lightning events and, on the other hand, optical outputs (or lack thereof) of the same discharge process. This is done, first, using coordinated very high frequency (VHF) and optical observations from the FORTE satellite and, second, using coordinated sferic and all-sky optical observations from the Los Alamos Sferic Array. In both cases, it is found that the sought coincidences are exceedingly rare. Moreover, in the handful of coincidences between optical and intense radio emissions that have been identified, the radio emissions differ from their usual behavior, by being accompanied by approximately simultaneous "conventional" lightning radio emissions. It is implied that the most radio-powerful intracloud emission process essentially differs from ordinary incandescent lightning. C1 [Jacobson, A. R.] Univ Washington, Washington, DC USA. [Light, T. E. L.; Hamlin, T.; Nemzek, R.] Los Alamos Natl Lab, ISR 2, Los Alamos, NM USA. RP Jacobson, AR (reprint author), Univ Washington, Washington, DC USA. EM abramj@u.washington.edu FU National Science Foundation [0947130]; Defense Advanced Research Projects Agency's Nimbus program; US Department of Energy FX One author (ARJ) was supported in this work by National Science Foundation grant 0947130 and by the Defense Advanced Research Projects Agency's Nimbus program, led by Dr. Matthew Goodman. The other authors contributed under the auspices of the US Department of Energy. NR 56 TC 4 Z9 5 U1 0 U2 8 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 0992-7689 J9 ANN GEOPHYS-GERMANY JI Ann. Geophys. PY 2013 VL 31 IS 3 BP 563 EP 580 DI 10.5194/angeo-31-563-2013 PG 18 WC Astronomy & Astrophysics; Geosciences, Multidisciplinary; Meteorology & Atmospheric Sciences SC Astronomy & Astrophysics; Geology; Meteorology & Atmospheric Sciences GA 137JQ UT WOS:000318432300016 ER PT S AU Hentschinski, M Vera, AS Salas, C AF Hentschinski, M. Sabio Vera, Agustin Salas, Clara BE Capua, M Fiore, R Papa, A Vera, AS Tassi, E TI The hard to soft Pomeron transition in small x DIS data using optimal renormalization SO DIFFRACTION 2012 SE AIP Conference Proceedings LA English DT Proceedings Paper CT International Workshop on Diffraction in High Energy Physics (DIFFRACTION) CY SEP 10-15, 2012 CL Puerto del Carmen, SPAIN SP LHCPhenoNet, Inst Fisica Teorica, Univ Autonoma Madrid, Ist Nazl Fisica Nucl, Univ Calabria, CERN, Univ Calabria, Phys Dept, INFN, Autonoma Univ, Inst Theoret Phys (IFT UAM/CSIC), DESY, LHC Era, European Network Adv Phenomenol (LHCPhenoNet) DE High energy resummation; Pomeron intercept ID APPROXIMATION AB We show that it is possible to describe the effective Pomeron intercept, determined from the HERA Deep Inelastic Scattering data at small values of Bjorken x, using next-to-leading order BFKL evolution together with collinear improvements. To obtain a good description over the whole range of Q(2) we use a non-Abelian physical renormalization scheme with BLM optimal scale, combined with a parametrization of the running coupling in the infrared region. C1 [Hentschinski, M.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Hentschinski, M (reprint author), Brookhaven Natl Lab, Upton, NY 11973 USA. RI Hentschinski, Martin/A-9708-2015 OI Hentschinski, Martin/0000-0003-2922-7308 NR 14 TC 0 Z9 0 U1 0 U2 0 PU AMER INST PHYSICS PI MELVILLE PA 2 HUNTINGTON QUADRANGLE, STE 1NO1, MELVILLE, NY 11747-4501 USA SN 0094-243X BN 978-0-7354-1146-3 J9 AIP CONF PROC PY 2013 VL 1523 BP 59 EP 62 DI 10.1063/1.4802116 PG 4 WC Physics, Particles & Fields SC Physics GA BES95 UT WOS:000317985000014 ER PT S AU Fazio, S AF Fazio, Salvatore BE Capua, M Fiore, R Papa, A Vera, AS Tassi, E TI GPDs at an Electron Ion Collider SO DIFFRACTION 2012 SE AIP Conference Proceedings LA English DT Proceedings Paper CT International Workshop on Diffraction in High Energy Physics (DIFFRACTION) CY SEP 10-15, 2012 CL Puerto del Carmen, SPAIN SP LHCPhenoNet, Inst Fisica Teorica, Univ Autonoma Madrid, Ist Nazl Fisica Nucl, Univ Calabria, CERN, Univ Calabria, Phys Dept, INFN, Autonoma Univ, Inst Theoret Phys (IFT UAM/CSIC), DESY, LHC Era, European Network Adv Phenomenol (LHCPhenoNet) DE GPDs; DVCS; VMP; EIC AB The feasibility for a precise determination of Generalized Parton Distribution (GPDs) functions at an Electron Ion Collider (EIC) has been explored. The high luminosity of the machine, together with the large resolution and rapidity acceptance of the new dedicated detector, will open opportunity for high precision measurements of GPDs. We report on the study of GPDs from deeply virtual Compton scattering (DVCS). We also point out that such measurements at a proposed EIC provide insight to both, the transverse distribution of sea quarks and gluons as well as the proton spin decomposition. C1 Brookhaven Natl Lab, Upton, NY 11973 USA. RP Fazio, S (reprint author), Brookhaven Natl Lab, Upton, NY 11973 USA. RI Fazio, Salvatore /G-5156-2010 NR 4 TC 0 Z9 0 U1 0 U2 2 PU AMER INST PHYSICS PI MELVILLE PA 2 HUNTINGTON QUADRANGLE, STE 1NO1, MELVILLE, NY 11747-4501 USA SN 0094-243X BN 978-0-7354-1146-3 J9 AIP CONF PROC PY 2013 VL 1523 BP 79 EP 82 DI 10.1063/1.4802121 PG 4 WC Physics, Particles & Fields SC Physics GA BES95 UT WOS:000317985000019 ER PT S AU Guryn, W AF Guryn, Wlodek CA STAR Collaboration BE Capua, M Fiore, R Papa, A Vera, AS Tassi, E TI Transverse spin asymmetries in the CNI region in polarized proton-proton elastic scattering at STAR SO DIFFRACTION 2012 SE AIP Conference Proceedings LA English DT Proceedings Paper CT International Workshop on Diffraction in High Energy Physics (DIFFRACTION) CY SEP 10-15, 2012 CL Puerto del Carmen, SPAIN SP LHCPhenoNet, Inst Fisica Teorica, Univ Autonoma Madrid, Ist Nazl Fisica Nucl, Univ Calabria, CERN, Univ Calabria, Phys Dept, INFN, Autonoma Univ, Inst Theoret Phys (IFT UAM/CSIC), DESY, LHC Era, European Network Adv Phenomenol (LHCPhenoNet) DE Polarization; Elastic Scattering ID 1ST MEASUREMENT; ROOT-S=200 GEV AB We shall present the result on single spin asymmetry (A(N)) in polarized proton-proton scattering at root s = 200 GeV in small four momentum transferred squared (t) region. With the Roman Pots of the pp2pp experiment, installed at the STAR detector at RHIC, a data sample of about 20 million elastic events in -t range of 0.003 <= vertical bar t vertical bar <= 0.035 (GeV/c)(2) was analyzed. A fit of t-dependence of A(N) indicates that a hadronic spin-flip amplitude is comparable to zero. C1 [Guryn, Wlodek; STAR Collaboration] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Guryn, W (reprint author), Brookhaven Natl Lab, Upton, NY 11973 USA. NR 12 TC 0 Z9 0 U1 0 U2 0 PU AMER INST PHYSICS PI MELVILLE PA 2 HUNTINGTON QUADRANGLE, STE 1NO1, MELVILLE, NY 11747-4501 USA SN 0094-243X BN 978-0-7354-1146-3 J9 AIP CONF PROC PY 2013 VL 1523 BP 194 EP 198 DI 10.1063/1.4802148 PG 5 WC Physics, Particles & Fields SC Physics GA BES95 UT WOS:000317985000046 ER PT S AU Van Buren, G AF Van Buren, G. CA STAR Collaboration BE Capua, M Fiore, R Papa, A Vera, AS Tassi, E TI STAR: Characterizing Hot Quark Matter SO DIFFRACTION 2012 SE AIP Conference Proceedings LA English DT Proceedings Paper CT International Workshop on Diffraction in High Energy Physics (DIFFRACTION) CY SEP 10-15, 2012 CL Puerto del Carmen, SPAIN SP LHCPhenoNet, Inst Fisica Teorica, Univ Autonoma Madrid, Ist Nazl Fisica Nucl, Univ Calabria, CERN, Univ Calabria, Phys Dept, INFN, Autonoma Univ, Inst Theoret Phys (IFT UAM/CSIC), DESY, LHC Era, European Network Adv Phenomenol (LHCPhenoNet) DE relativistic heavy ion collisions; quark gluon plasma AB With discovery of Quark Gluon Plasma well-established at RHIC, the STAR Experiment continues to work toward a more complete understanding of properties of the produced matter, and the conditions necessary for the phase change. We will present recent progress on characterizing quark matter at high temperature through a wide variety of measurement techniques in STAR's repertoire: from observing species suppression and correlations, to determining statistical moments and prospecting for symmetry-breaking. RHIC has further embarked on a program to study this matter through a range of conditions achieved by varying the collision energies, which are hoped to span and locate the QCD critical point. We will show how STAR's toolkit is already providing intriguing results from the the first phase of this program and discuss possible future directions for the program. C1 [Van Buren, G.; STAR Collaboration] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Van Buren, G (reprint author), Brookhaven Natl Lab, POB 5000, Upton, NY 11973 USA. NR 21 TC 0 Z9 0 U1 0 U2 2 PU AMER INST PHYSICS PI MELVILLE PA 2 HUNTINGTON QUADRANGLE, STE 1NO1, MELVILLE, NY 11747-4501 USA SN 0094-243X BN 978-0-7354-1146-3 J9 AIP CONF PROC PY 2013 VL 1523 BP 216 EP 220 DI 10.1063/1.4802153 PG 5 WC Physics, Particles & Fields SC Physics GA BES95 UT WOS:000317985000051 ER PT S AU Hentschinski, M Murdaca, B AF Hentschinski, Martin Murdaca, Beatrice BE Capua, M Fiore, R Papa, A Vera, AS Tassi, E TI The Mueller-Tang jet impact factor at NLO from the high energy effective action SO DIFFRACTION 2012 SE AIP Conference Proceedings LA English DT Proceedings Paper CT International Workshop on Diffraction in High Energy Physics (DIFFRACTION) CY SEP 10-15, 2012 CL Puerto del Carmen, SPAIN SP LHCPhenoNet, Inst Fisica Teorica, Univ Autonoma Madrid, Ist Nazl Fisica Nucl, Univ Calabria, CERN, Univ Calabria, Phys Dept, INFN, Autonoma Univ, Inst Theoret Phys (IFT UAM/CSIC), DESY, LHC Era, European Network Adv Phenomenol (LHCPhenoNet) DE High energy effective action; jets with rapidity gaps; diffraction; BFKL ID QCD EFFECTIVE ACTION; SCATTERING AB We report on recent progress in the evaluation of next-to-leading order observables using Lipatov's QCD high energy effective action. In this contribution we focus on the determination of the real part of the next-to-leading order corrections to the Mueller-Tang impact factor which is the only missing element for a complete NLO BFKL description of quark induced dijet events with a rapidity gap. C1 [Hentschinski, Martin] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Murdaca, Beatrice] Univ Calabria, Dipartimento Fis, I-87030 Commenda Di Rende, Italy. [Murdaca, Beatrice] Ist Nazl Fis Nucleare, Grp Coll Cosenza, I-87036 Cosenza, Italy. RP Hentschinski, M (reprint author), Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. RI Hentschinski, Martin/A-9708-2015; OI Hentschinski, Martin/0000-0003-2922-7308; Murdaca, Beatrice/0000-0002-1681-5998 FU U.S. Department of Energy [DE-AC02-98CH10886]; Department of Energy [DE-AC02-98CH10886]; BNL "Laboratory Directed Research and Development" [LDRD 12-034] FX We would like to thank G. Chachamis, J. Madrigal Martinez and A. Sabio Vera for fruit-ful collaboration. M.H. acknowledges support from the U.S. Department of Energy under contract number DE-AC02-98CH10886 and a BNL Laboratory Directed Research and Development grant (LDRD 12-034). NR 28 TC 0 Z9 0 U1 0 U2 3 PU AMER INST PHYSICS PI MELVILLE PA 2 HUNTINGTON QUADRANGLE, STE 1NO1, MELVILLE, NY 11747-4501 USA SN 0094-243X BN 978-0-7354-1146-3 J9 AIP CONF PROC PY 2013 VL 1523 BP 268 EP + DI 10.1063/1.4802164 PG 2 WC Physics, Particles & Fields SC Physics GA BES95 UT WOS:000317985000062 ER PT S AU Balitsky, I AF Balitsky, Ian BE Capua, M Fiore, R Papa, A Vera, AS Tassi, E TI Photon impact factor in the NLO SO DIFFRACTION 2012 SE AIP Conference Proceedings LA English DT Proceedings Paper CT International Workshop on Diffraction in High Energy Physics (DIFFRACTION) CY SEP 10-15, 2012 CL Puerto del Carmen, SPAIN SP LHCPhenoNet, Inst Fisica Teorica, Univ Autonoma Madrid, Ist Nazl Fisica Nucl, Univ Calabria, CERN, Univ Calabria, Phys Dept, INFN, Autonoma Univ, Inst Theoret Phys (IFT UAM/CSIC), DESY, LHC Era, European Network Adv Phenomenol (LHCPhenoNet) DE High energy; Conformal invariance; Wilson lines ID EVOLUTION AB The photon impact factor for the BFKL pomeron is calculated in the next-to-leading order (NLO) approximation using the operator expansion in Wilson lines. The result is represented as a NLO k(T)-factorization formula for the structure functions of small-x deep inelastic scattering. C1 JLab, Newport News, VA 23606 USA. RP Balitsky, I (reprint author), JLab, 12000 Jefferson Ave, Newport News, VA 23606 USA. NR 20 TC 0 Z9 0 U1 0 U2 1 PU AMER INST PHYSICS PI MELVILLE PA 2 HUNTINGTON QUADRANGLE, STE 1NO1, MELVILLE, NY 11747-4501 USA SN 0094-243X BN 978-0-7354-1146-3 J9 AIP CONF PROC PY 2013 VL 1523 BP 276 EP 281 DI 10.1063/1.4802166 PG 6 WC Physics, Particles & Fields SC Physics GA BES95 UT WOS:000317985000064 ER PT S AU Albrow, MG AF Albrow, M. G. CA CDF Collaboration BE Capua, M Fiore, R Papa, A Vera, AS Tassi, E TI Central Exclusive Production of Hadrons in CDF SO DIFFRACTION 2012 SE AIP Conference Proceedings LA English DT Proceedings Paper CT International Workshop on Diffraction in High Energy Physics (DIFFRACTION) CY SEP 10-15, 2012 CL Puerto del Carmen, SPAIN SP LHCPhenoNet, Inst Fisica Teorica, Univ Autonoma Madrid, Ist Nazl Fisica Nucl, Univ Calabria, CERN, Univ Calabria, Phys Dept, INFN, Autonoma Univ, Inst Theoret Phys (IFT UAM/CSIC), DESY, LHC Era, European Network Adv Phenomenol (LHCPhenoNet) DE Diffraction; Double pomeron exchange; Central exclusive production AB At the Fermilab Tevatron with root s = 900 and 1960 GeV, we have studied exclusive double pomeron exchange in the Collider Detector at Fermilab, CDF. With similar to 300,000 events we present the mass spectrum of two hadrons, h(+)h(-), assumed to be pions, with vertical bar eta(pi)vertical bar < 1.3 and two rapidity gaps Delta eta > 4.6. The mass spectrum shows resonance structures, including f(0)(980), f(2)(1270), and f(0)(1370). The cross section ratio 1960 GeV/900 GeV and the mean p(T) (pair) show mass-dependent structures, even above M = 2 GeV where there are no established pi(+)pi(-) resonances. The data extend above M = 5 GeV. We place an upper limit on exclusive chi(c0) -> pi(+)pi(-) and K+K-. C1 Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. RP Albrow, MG (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. NR 7 TC 0 Z9 0 U1 0 U2 0 PU AMER INST PHYSICS PI MELVILLE PA 2 HUNTINGTON QUADRANGLE, STE 1NO1, MELVILLE, NY 11747-4501 USA SN 0094-243X BN 978-0-7354-1146-3 J9 AIP CONF PROC PY 2013 VL 1523 BP 294 EP 297 DI 10.1063/1.4802170 PG 4 WC Physics, Particles & Fields SC Physics GA BES95 UT WOS:000317985000068 ER PT S AU Albrow, MG AF Albrow, Michael G. BE Capua, M Fiore, R Papa, A Vera, AS Tassi, E TI High Precision Spectrometers for Very Forward Protons in CMS SO DIFFRACTION 2012 SE AIP Conference Proceedings LA English DT Proceedings Paper CT International Workshop on Diffraction in High Energy Physics (DIFFRACTION) CY SEP 10-15, 2012 CL Puerto del Carmen, SPAIN SP LHCPhenoNet, Inst Fisica Teorica, Univ Autonoma Madrid, Ist Nazl Fisica Nucl, Univ Calabria, CERN, Univ Calabria, Phys Dept, INFN, Autonoma Univ, Inst Theoret Phys (IFT UAM/CSIC), DESY, LHC Era, European Network Adv Phenomenol (LHCPhenoNet) DE Higgs; Central exclusive production AB We plan to add proton tracking and timing detectors at z = 240-250 m on both sides of CMS to study central exclusive production, with one or both protons measured, and single diffraction. They provide measurements of p + p -> p + X + p, where X = Z,H,W+W- and multiparticle states (with or without jets), as well as single high mass diffraction in low pile-up runs. C1 Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. RP Albrow, MG (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. NR 10 TC 0 Z9 0 U1 0 U2 0 PU AMER INST PHYSICS PI MELVILLE PA 2 HUNTINGTON QUADRANGLE, STE 1NO1, MELVILLE, NY 11747-4501 USA SN 0094-243X BN 978-0-7354-1146-3 J9 AIP CONF PROC PY 2013 VL 1523 BP 320 EP 323 DI 10.1063/1.4802177 PG 4 WC Physics, Particles & Fields SC Physics GA BES95 UT WOS:000317985000075 ER PT S AU Rajamanickam, S Boman, EG AF Rajamanickam, Sivasankaran Boman, Erik G. BE Bader, DA Meyerhenke, H Sanders, P Wagner, D TI Parallel partitioning with Zoltan: Is hypergraph partitioning worth it? SO GRAPH PARTITIONING AND GRAPH CLUSTERING SE Contemporary Mathematics LA English DT Proceedings Paper CT 10th DIMACS Implementation Challenge Workshop CY FEB 13-14, 2012 CL Georgia Inst Technol, Atlanta, GA SP DIMACS, Command Control & Interoperabil Ctr Adv Data Anal, Pacific NW Natl Lab, Sandia Natl Lab, Intel Corp, Deutsch Forschungsgemeinschaft HO Georgia Inst Technol DE Graph partitioning; hypergraph partitioning; parallel computing ID MATRIX-VECTOR MULTIPLICATION AB Graph partitioning is an important and well studied problem in combinatorial scientific computing, and is commonly used to reduce communication in parallel computing. Different models (graph, hypergraph) and objectives (edge cut, boundary vertices) have been proposed. Hypergraph partitioning has become increasingly popular over the last decade. Its main strength is that it accurately captures communication volume, but it is slower to compute than graph partitioning. We present an empirical study of the Zoltan parallel hypergraph and graph (PEG) partitioner on graphs from the 10th DIMACS implementation challenge and some directed (nonsymmetric) graphs. We show that hypergraph partitioning is superior to graph partitioning on directed graphs (nonsymmetric matrices), where the communication volume is reduced in several cases by over an order of magnitude, but has no significant benefit on undirected graphs (symmetric matrices) using current parallel software tools. C1 [Rajamanickam, Sivasankaran; Boman, Erik G.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Rajamanickam, S (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM srajama@sandia.gov; egboman@sandia.gov NR 22 TC 1 Z9 1 U1 0 U2 8 PU AMER MATHEMATICAL SOC PI PROVIDENCE PA P.O. BOX 6248, PROVIDENCE, RI 02940 USA SN 0271-4132 BN 978-0-8218-9038-7 J9 CONTEMP MATH PY 2013 VL 588 BP 37 EP 52 DI 10.1090/conm/588/11711 PG 16 WC Mathematics SC Mathematics GA BES46 UT WOS:000317939900004 ER PT S AU Buluc, A Madduri, K AF Buluc, Aydin Madduri, Kamesh BE Bader, DA Meyerhenke, H Sanders, P Wagner, D TI Graph partitioning for scalable distributed graph computations SO GRAPH PARTITIONING AND GRAPH CLUSTERING SE Contemporary Mathematics LA English DT Proceedings Paper CT 10th DIMACS Implementation Challenge Workshop CY FEB 13-14, 2012 CL Georgia Inst Technol, Atlanta, GA SP DIMACS, Command Control & Interoperabil Ctr Adv Data Anal, Pacific NW Natl Lab, Sandia Natl Labs, Intel Corp, Deutsch Forschungsgemeinschaft HO Georgia Inst Technol DE graph partitioning; hypergraph partitioning; inter-node communication modeling; breadth-first search; 2D decomposition AB Inter-node communication time constitutes a significant fraction of the execution time of graph algorithms on distributed-memory systems. Global computations on large-scale sparse graphs with skewed degree distributions are particularly challenging to optimize for, as prior work shows that it is difficult to obtain balanced partitions with low edge cuts for these graphs. In this work, we attempt to determine the optimal partitioning and distribution of such graphs, for load-balanced parallel execution of communication-intensive graph algorithms. We use breadth-first search (BFS) as a representative example, and derive upper bounds on the communication costs incurred with a two-dimensional partitioning of the graph. We present empirical results for communication costs with various graph partitioning strategies, and also obtain parallel BFS execution times for several large-scale DIMACS Challenge instances on a supercomputing platform. Our performance results indicate that for several graph instances, reducing work and communication imbalance among partitions is more important than minimizing the total edge cut. C1 [Buluc, Aydin] Lawrence Berkeley Natl Lab, Berkeley, CA USA. [Madduri, Kamesh] Penn State Univ, State Coll, PA 16801 USA. RP Buluc, A (reprint author), Lawrence Berkeley Natl Lab, Berkeley, CA USA. FU Office of Science, U.S. Department of Energy [DE-ACO2-05CH11231] FX This work was supported by the Director, Office of Science, U.S. Department of Energy under Contract No. DE-ACO2-05CH11231. NR 10 TC 2 Z9 2 U1 0 U2 2 PU AMER MATHEMATICAL SOC PI PROVIDENCE PA P.O. BOX 6248, PROVIDENCE, RI 02940 USA SN 0271-4132 BN 978-0-8218-9038-7 J9 CONTEMP MATH PY 2013 VL 588 BP 83 EP + DI 10.1090/conm/588/11709 PG 3 WC Mathematics SC Mathematics GA BES46 UT WOS:000317939900007 ER PT S AU Djidjev, H Onus, M AF Djidjev, Hristo Onus, Melih BE Bader, DA Meyerhenke, H Sanders, P Wagner, D TI Using graph partitioning for efficient network modularity optimization SO GRAPH PARTITIONING AND GRAPH CLUSTERING SE Contemporary Mathematics LA English DT Proceedings Paper CT 10th DIMACS Implementation Challenge Workshop CY FEB 13-14, 2012 CL Georgia Inst Technol, Atlanta, GA SP DIMACS, Command Control & Interoperabil Ctr Adv Data Anal, Pacific NW Natl Lab, Sandia Natl Labs, Intel Corp, Deutsch Forschungsgemeinschaft HO Georgia Inst Technol ID COMMUNITY; DYNAMICS AB The paper reviews an approach for finding the communities of a network developed by the authors [WAW'06, Lecture Notes in Computer Science, Volume 4936/2008, 117-128, IEEE TPDS vol. PP, issue 99, 2012], which is based on a reduction of the modularity optimization problem to the minimum weighted cut problem, and gives an experimental evaluation of an implementation based on that approach on graphs from the 10th DIMACS Implementation Challenge Testbed. Specifically, we describe a reduction from the problem of finding a partition of the nodes of a graph G that maximizes the modularity to the problem of finding a partition that minimizes the weight of the cut in a complete graph on the same node set as G, and weights dependent on a random graph model associated with G. The resulting minimum cut problem can then be solved by modifying existing codes for graph partitioning. We compare the performance of our implementation based on the Metis graph partitioning tool [SIAM J. Sci. Comp. 20, 359-392] against one of the best performing algorithms described in this volume. C1 [Djidjev, Hristo] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. [Onus, Melih] Bilkent Univ, Dept Comp Engn, TR-06800 Ankara, Turkey. RP Djidjev, H (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. FU Department of Energy [W-705-ENG-36]; Los Alamos National Laboratory Directed Research and Development Program (LDRD) [20110093DR, 20130252ER] FX The work of the first author has been supported by the Department of Energy under contract W-705-ENG-36 and by the Los Alamos National Laboratory Directed Research and Development Program (LDRD), projects 20110093DR and 20130252ER. NR 34 TC 0 Z9 0 U1 1 U2 3 PU AMER MATHEMATICAL SOC PI PROVIDENCE PA P.O. BOX 6248, PROVIDENCE, RI 02940 USA SN 0271-4132 BN 978-0-8218-9038-7 J9 CONTEMP MATH PY 2013 VL 588 BP 103 EP + DI 10.1090/conm/588/11713 PG 4 WC Mathematics SC Mathematics GA BES46 UT WOS:000317939900008 ER PT J AU Grover, S Teplin, CW Li, JV Bobela, DC Bornstein, J Schroeter, P Johnston, S Guthrey, H Stradins, P Branz, HM Young, DL AF Grover, Sachit Teplin, Charles W. Li, Jian V. Bobela, David C. Bornstein, Jon Schroeter, Paul Johnston, Steve Guthrey, Harvey Stradins, Paul Branz, Howard M. Young, David L. TI Device Physics of Heteroepitaxial Film c-Si Heterojunction Solar Cells SO IEEE JOURNAL OF PHOTOVOLTAICS LA English DT Article DE Charge recombination; diode ideality factor; heteroepitaxial silicon; open-circuit voltage; photovoltaic (PV) cells; quantum efficiency (QE) ID POLYCRYSTALLINE SILICON; SURFACE-RECOMBINATION; CHALLENGES; EFFICIENCY; GLASS AB We characterize heterojunction solar cells made from single-crystal silicon films grown heteroepitaxially using hot-wire chemical vapor deposition (HWCVD). Heteroepitaxy-induced dislocations limit the cell performance, providing a unique platform to study the device physics of thin crystal Si heterojunction solar cells. Hydrogen passivation of these dislocations enables an open-circuit voltage V-OC close to 580 mV. However, dislocations are partially active, even after passivation. Using standard characterization methods, we compare the performance of heteroepitaxial absorbers with homoepitaxial absorbers that are free of dislocations. Heteroepitaxial cells have a smaller diffusion length and a larger ideality factor, indicating stronger recombination, which leads to inefficient current collection and a lower V-OC than homoepitaxial cells. Modeling indicates that the recombination in the inversion layer of heterojunction cells made from defective absorbers is comparable with the overall recombination in the bulk. Temperature-dependent V-OC measurements point to significant recombination at the interface that is attributable to the presence of dislocations. C1 [Grover, Sachit; Teplin, Charles W.; Li, Jian V.; Johnston, Steve; Guthrey, Harvey; Stradins, Paul; Branz, Howard M.; Young, David L.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Bobela, David C.; Bornstein, Jon; Schroeter, Paul] Ampulse Corp, Golden, CO 80401 USA. RP Grover, S (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM sachit.grover@nrel.gov; Charles.Teplin@NREL.gov; jian.li@nrel.gov; David@ampulse.com; jon@ampulse.com; Paul@ampulse.com; steve.johnston@nrel.gov; harvey.guthrey@nrel.gov; pauls.stradins@nrel.gov; howard.branz@nrel.gov; David.Young@nrel.gov RI Grover, Sachit/M-1881-2013; Li, Jian/B-1627-2016 FU U.S. Department of Energy Solar Energy Technologies Program [AC36-08-GO28308]; Ampulse Corporation FX This work was supported by the U.S. Department of Energy Solar Energy Technologies Program under Contract AC36-08-GO28308 and by the Ampulse Corporation. NR 27 TC 8 Z9 8 U1 1 U2 26 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 2156-3381 J9 IEEE J PHOTOVOLT JI IEEE J. Photovolt. PD JAN PY 2013 VL 3 IS 1 BP 230 EP 235 DI 10.1109/JPHOTOV.2012.2223455 PG 6 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA 137KF UT WOS:000318434000036 ER PT J AU Hacke, P Smith, R Terwilliger, K Glick, S Jordan, D Johnston, S Kempe, M Kurtz, S AF Hacke, Peter Smith, Ryan Terwilliger, Kent Glick, Stephen Jordan, Dirk Johnston, Steve Kempe, Michael Kurtz, Sarah TI Testing and Analysis for Lifetime Prediction of Crystalline Silicon PV Modules Undergoing Degradation by System Voltage Stress SO IEEE JOURNAL OF PHOTOVOLTAICS LA English DT Article DE Current-voltage (I-V) characteristics; degradation; high-voltage techniques; photovoltaic (PV) cells; photovoltaic systems; reliability ID PHOTOVOLTAIC MODULES; FAILURE AB Acceleration factors are calculated for crystalline silicon photovoltaic modules under system voltage stress by comparing the module power during degradation outdoors with that in accelerated testing at three temperatures and 85% relative humidity. A lognormal analysis is applied to the accelerated lifetime test data, considering failure at 80% of the initial module power. Activation energy of 0.73 eV for the rate of failure is determined for the chamber testing at constant relative humidity, and the probability of module failure at an arbitrary temperature is predicted. To obtain statistical data for multiple modules over the course of degradation in situ of the test chamber, dark I-V measurements are obtained and transformed using superposition, which is found to be well suited for rapid and quantitative evaluation of potential-induced degradation. It is determined that shunt resistance measurements alone do not represent the extent of power degradation. This is explained with a two-diode model analysis that shows an increasing second diode recombination current and ideality factor as the degradation in module power progresses. Failure modes of the modules stressed outdoors are examined and compared with those stressed in accelerated tests. C1 [Hacke, Peter; Smith, Ryan; Terwilliger, Kent; Glick, Stephen; Jordan, Dirk; Johnston, Steve; Kempe, Michael; Kurtz, Sarah] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Hacke, P (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM peter.hacke@nrel.gov; Ryan.Smith@nrel.gov; kent.terwilliger@nrel.gov; Stephen.Glick@nrel.gov; dirk.jordan@nrel.gov; steve.johnston@nrel.gov; Michael.Kempe@nrel.gov; Sarah.Kurtz@nrel.gov FU U.S. Department of Energy [DE-AC36-08-GO28308]; National Renewable Energy Laboratory FX This work was supported by the U.S. Department of Energy under Contract DE-AC36-08-GO28308 with the National Renewable Energy Laboratory. NR 32 TC 22 Z9 24 U1 3 U2 38 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 2156-3381 J9 IEEE J PHOTOVOLT JI IEEE J. Photovolt. PD JAN PY 2013 VL 3 IS 1 BP 246 EP 253 DI 10.1109/JPHOTOV.2012.2222351 PG 8 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA 137KF UT WOS:000318434000038 ER PT J AU Pattnaik, S Xiao, T Shinar, R Shinar, J Dalal, VL AF Pattnaik, Sambit Xiao, Teng Shinar, R. Shinar, J. Dalal, V. L. TI Novel Hybrid Amorphous/Organic Tandem Junction Solar Cell SO IEEE JOURNAL OF PHOTOVOLTAICS LA English DT Article DE Amorphous semiconductors; degradation; organic semiconductors; photovoltaic (PV) cells; silicon ID MICROCRYSTALLINE SILICON; POLYMER; TRANSPORT AB We report on a novel hybrid amorphous Si-organic series-connected tandem junction solar cell. The solar cell is fabricated on indium tin oxide (ITO)-coated glass and uses an a-(Si,C):H as the first cell and a P3HT/PCBM organic cell as the second cell. An intermediate ITO layer is used as an ohmic layer which provides an excellent contact to both the first and the second cells. By adjusting the bandgap and thickness of the first a-(Si,C):H cell, we achieve an almost complete matching of currents produced by the first and the second cells. The first cell produces similar to 0.95-1.0-V open-circuit voltage, and the second cell produces similar to 0.6-V open-circuit voltage. The combined cell produces 1.5-V open-circuit voltage and had a fill factor of 77%, showing the effectiveness of the intermediate ITO layer to act as an excellent connecting layer between the two cells. When such an ITO layer is not used, the fill factor is very poor. The solar conversion efficiency of the organic cell was 4.3%, whereas the efficiency of the tandem cell was 5.7%. We also measured the stability of the organic cell with and without an inorganic cell acting as a filter in front. It is shown that the degradation of the organic cell is much higher when it is subjected to a full solar spectrum, as compared with when it is subjected to light passing through an inorganic cell first, which filters out ultraviolet (UV) and blue photons. Thus, we show that this new cell combination has the potential to significantly increase the efficiency of organic cells while also decreasing the instability. We also discuss the potential of achieving much higher efficiencies, that is approaching 20%, by using an appropriate combination of amorphous and organic cells. An example is shown next. C1 [Pattnaik, Sambit; Shinar, R.; Dalal, V. L.] Iowa State Univ, Microelect Res Ctr, Ames, IA 50011 USA. [Pattnaik, Sambit; Shinar, R.; Dalal, V. L.] Iowa State Univ, Dept Elect & Comp Engn, Ames, IA 50011 USA. [Xiao, Teng; Shinar, J.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Xiao, Teng; Shinar, J.] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. RP Pattnaik, S (reprint author), Iowa State Univ, Microelect Res Ctr, Ames, IA 50011 USA. EM pattnaik@iastate.edu; txiao@iastate.edu; rshinar@iastate.edu; shinar@ameslab.gov; vdalal@iastate.edu FU National Science Foundation; Iowa Power Fund; U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division [DE-AC 02-07CH11358] FX This work was supported by the National Science Foundation and Iowa Power Fund for some of the work. This work was also supported in part by the U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division, under Contract DE-AC 02-07CH11358. NR 20 TC 5 Z9 5 U1 0 U2 39 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 2156-3381 J9 IEEE J PHOTOVOLT JI IEEE J. Photovolt. PD JAN PY 2013 VL 3 IS 1 BP 295 EP 299 DI 10.1109/JPHOTOV.2012.2212700 PG 5 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA 137KF UT WOS:000318434000046 ER PT J AU Ray, B Khan, MR Black, C Alam, MA AF Ray, Biswajit Khan, Mohammad Ryyan Black, Charles Alam, Muhammad Ashraful TI Nanostructured Electrodes for Organic Solar Cells: Analysis and Design Fundamentals SO IEEE JOURNAL OF PHOTOVOLTAICS LA English DT Article DE Bulk heterojunction (BHJ); fill factor (FF); morphology; nanostructured electrodes (NEs); organic photovoltaic (OPV) cell ID POWER CONVERSION EFFICIENCY; POLYMER PHOTOVOLTAIC CELLS; RECOMBINATION; BLENDS; POLY(3-HEXYLTHIOPHENE); HETEROJUNCTIONS; ENHANCEMENT; PERFORMANCE; MORPHOLOGY; NETWORK AB Nanostructured electrodes (NEs) improve optical absorption and charge collection in photovoltaic (PV) devices. Traditionally, the electrodes have been designed exclusively for higher optical absorption. Such an optical design of the electrodes does not necessarily ensure better charge collection. Since the efficiency of organic PV (OPV) devices is hindered by the low carrier mobility of the organic semiconductors, the charge collection property of the NEs provides an interesting design alternative. The goal of this paper is the formulation of the essential design rules for NEs to improve charge collection in the low-mobility organic materials. We use detailed optoelectronic device simulation to explore the physics of NEs embedded in the organic semiconductors and quantify its effect on the performance gain of organic solar cells. Our analysis suggests that an optimum codesign of electrodes and morphology is essential for significant performance improvement (mainly through fill factor) in OPV cells. C1 [Ray, Biswajit; Khan, Mohammad Ryyan; Alam, Muhammad Ashraful] Purdue Univ, Sch Elect & Comp Engn, W Lafayette, IN 47906 USA. [Black, Charles] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Ray, B (reprint author), Purdue Univ, Sch Elect & Comp Engn, W Lafayette, IN 47906 USA. EM biswajit.025@gmail.com; ryyan.khan.eee@gmail.com; ctblack@bnl.gov; alam@purdue.edu FU Center for Re-Defining Photovoltaic Efficiency Through Molecule Scale Control, an Energy Frontier Research Center; U.S. Department of Energy Office of Science; Office of Basic Energy Sciences [DE-SC0001085]; Network of Computational Nanotechnology from the National Science Foundation [EEC-0228390] FX This work was supported in part by the Center for Re-Defining Photovoltaic Efficiency Through Molecule Scale Control, an Energy Frontier Research Center funded by the U.S. Department of Energy Office of Science, and in part by the Office of Basic Energy Sciences under Award DE-SC0001085. The computational resources for this work were provided by the Network of Computational Nanotechnology under Award EEC-0228390 from the National Science Foundation. NR 49 TC 11 Z9 11 U1 0 U2 27 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 2156-3381 J9 IEEE J PHOTOVOLT JI IEEE J. Photovolt. PD JAN PY 2013 VL 3 IS 1 BP 318 EP 329 DI 10.1109/JPHOTOV.2012.2220529 PG 12 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA 137KF UT WOS:000318434000049 ER PT J AU Ahrenkiel, RK Feldman, A Lehman, J Johnston, SW AF Ahrenkiel, R. K. Feldman, A. Lehman, J. Johnston, S. W. TI Novel Free-Carrier Pump-Probe Analysis of Carrier Transport in Semiconductors SO IEEE JOURNAL OF PHOTOVOLTAICS LA English DT Article DE Charge-carrier lifetime; free carrier absorption; photoconductive decay AB We have developed a pump-probe configuration to measure the carrier lifetime using the transient free-carrier density. The free-carrier absorption varies as lambda(2) Delta n/mu, where lambda is 10.6 mu m in this paper. We measure the transient photoconductive decay that is proportional to Delta n (*) mu. The data product gives Delta alpha (*) Delta sigma similar to lambda(2) Delta n(t)(2). The mobility variation is nullified by multiplying the data from the two parallel measurements. From the product data, both Delta n(t) and mu(Delta n) can be determined. A large increase in Delta alpha and decrease in mu are observed and caused by space-charge effects in regions of high injection. These data show the unexpected and remarkable result that the lifetime is relatively constant up to an injection level of about three times the doping level. However, the mobility decreases by about a factor of six over the same injection range. C1 [Ahrenkiel, R. K.; Feldman, A.] Colorado Sch Mines, Golden, CO 80401 USA. [Ahrenkiel, R. K.; Johnston, S. W.] Natl Renewable Energy Lab, Golden, CO 80402 USA. [Feldman, A.; Lehman, J.] NIST, Boulder, CO 80302 USA. RP Ahrenkiel, RK (reprint author), Colorado Sch Mines, Golden, CO 80401 USA. EM rahren@mac.com; ari1127@gmail.com; lehman@boulder.nist.gov; steve.johnston@nrel.gov NR 7 TC 3 Z9 3 U1 1 U2 6 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 2156-3381 J9 IEEE J PHOTOVOLT JI IEEE J. Photovolt. PD JAN PY 2013 VL 3 IS 1 BP 348 EP 352 DI 10.1109/JPHOTOV.2012.2215581 PG 5 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA 137KF UT WOS:000318434000053 ER PT J AU Madaeni, SH Sioshansi, R Denholm, P AF Madaeni, Seyed Hossein Sioshansi, Ramteen Denholm, Paul TI Comparing Capacity Value Estimation Techniques for Photovoltaic Solar Power SO IEEE JOURNAL OF PHOTOVOLTAICS LA English DT Article DE Approximation techniques; capacity value; photovoltaic (PV) solar; reliability theory ID LOAD-CARRYING CAPABILITY; UNITED-STATES; WIND POWER AB In this paper, we estimate the capacity value of photovoltaic (PV) solar plants in the western U.S. Our results show that PV plants have capacity values that range between 52% and 93%, depending on location and sun-tracking capability. We further compare more robust but data- and computationally-intense reliability-based estimation techniques with simpler approximation methods. We show that if implemented properly, these techniques provide accurate approximations of reliability-based methods. Overall, methods that are based on the weighted capacity factor of the plant provide the most accurate estimate. We also examine the sensitivity of PV capacity value to the inclusion of sun-tracking systems. C1 [Madaeni, Seyed Hossein; Sioshansi, Ramteen] Ohio State Univ, Integrated Syst Engn Dept, Columbus, OH 43210 USA. [Denholm, Paul] Natl Renewable Energy Lab, Strateg Energy Anal Ctr, Golden, CO 80401 USA. RP Madaeni, SH (reprint author), Pacific Gas & Elect Co, Short Term Elect Supply Dept, San Francisco, CA 94105 USA. EM SHM8@pge.com; sioshansi.1@osu.edu; paul.denholm@nrel.gov FU U.S. Department of Energy [DE-AC36-08GO28308]; Alliance for Sustainable Energy, LLC [AGG-1-11946-01] FX Manuscript received July 18, 2012; accepted August 29, 2012. Date of publication September 28, 2012; date of current version December 19, 2012. This work was supported by the U.S. Department of Energy through prime contract DE-AC36-08GO28308 and by the Alliance for Sustainable Energy, LLC, through subcontract AGG-1-11946-01. The opinions expressed and conclusions reached are solely those of the authors and do not represent the official position of Pacific Gas and Electric Company. NR 32 TC 10 Z9 11 U1 2 U2 23 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 2156-3381 J9 IEEE J PHOTOVOLT JI IEEE J. Photovolt. PD JAN PY 2013 VL 3 IS 1 BP 407 EP 415 DI 10.1109/JPHOTOV.2012.2217114 PG 9 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA 137KF UT WOS:000318434000063 ER PT J AU Fthenakis, V Anctil, A AF Fthenakis, Vasilis Anctil, Annick TI Direct Te Mining: Resource Availability and Impact on Cumulative Energy Demand of CdTe PV Life Cycles SO IEEE JOURNAL OF PHOTOVOLTAICS LA English DT Article DE CdTe photovoltaics (PV); life-cycle assessments (LCAs); photovoltaic cells ID TECHNOLOGIES AB As the availability of tellurium (Te) is constrained by the production rate of its main parent compound (Cu), its potential supply to deploy CdTe photovoltaics (PV) merits investigation. Recently, Te-rich ores and gold-telluride mines have been discovered in several places throughout the world that will allow the economic recovery of Te, independent of the production of copper. In conventional CdTe life-cycle assessments, the environmental impacts of mining and smelting are typically allocated to all the coproducts on the basis of the products' physical amount or economic values. Consequently, directly mining Te from such ores potentially might increase the environmental burden of mining and smelting operations in the life cycle of CdTe PV systems. Other factors influencing the impacts of direct Te mining include the presence of additional coproducts (e.g., gold and silver), the relative contribution of Te to the life-cycle cumulative energy demand (CED) of CdTe PV, the proportion of directly mined Te content relative to the content of the Cu byproduct in the Te-supply chain, and end-of-life CdTe PV recycling. We estimated that the total CED would increase by 1% when 100% of the supply came from direct mining and by 0.7% if we assume a supply mixture representing the ratios of the reserves. C1 [Fthenakis, Vasilis] Columbia Univ, New York, NY 10027 USA. [Fthenakis, Vasilis; Anctil, Annick] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Fthenakis, V (reprint author), Columbia Univ, New York, NY 10027 USA. EM vmf@bnl.gov; aanctil@bnl.gov NR 16 TC 6 Z9 6 U1 2 U2 18 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 2156-3381 J9 IEEE J PHOTOVOLT JI IEEE J. Photovolt. PD JAN PY 2013 VL 3 IS 1 BP 433 EP 438 DI 10.1109/JPHOTOV.2012.2216860 PG 6 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA 137KF UT WOS:000318434000067 ER PT J AU Repins, IL Romero, MJ Li, JV Wei, SH Kuciauskas, D Jiang, CS Beall, C DeHart, C Mann, J Hsu, WC Teeter, G Goodrich, A Noufi, R AF Repins, Ingrid L. Romero, Manuel J. Li, Jian V. Wei, Su-Huai Kuciauskas, Darius Jiang, Chun-Sheng Beall, Carolyn DeHart, Clay Mann, Jonathan Hsu, Wan-Ching Teeter, Glenn Goodrich, Al Noufi, Rommel TI Kesterite Successes, Ongoing Work, and Challenges: A Perspective From Vacuum Deposition SO IEEE JOURNAL OF PHOTOVOLTAICS LA English DT Article DE Cu2ZnSnS4 (CZTS); earth; kesterite; photovoltaic; thin film ID FILM SOLAR-CELLS; THIN-FILMS; PHOTOVOLTAICS; CU2ZNSNSE4; EFFICIENCY; CZTS; AVAILABILITY AB Recent years have seen dramatic improvements in the performance of kesterite devices. The existence of devices of comparable performance, made by a number of different techniques, provides some new perspective on what characteristics are likely fundamental to the material. Here, we review progress in kesterite device fabrication, aspects of the film characteristics that have yet to be understood, and challenges in device development that remain for kesterites to contribute significantly to photovoltaic manufacturing. Performance goals, as well as characteristics of mid-gap defect density, free carrier density, surfaces, grain boundaries, grain-to-grain uniformity, and bandgap alloying are discussed. C1 [Repins, Ingrid L.; Romero, Manuel J.; Li, Jian V.; Wei, Su-Huai; Kuciauskas, Darius; Jiang, Chun-Sheng; Beall, Carolyn; DeHart, Clay; Mann, Jonathan; Teeter, Glenn; Goodrich, Al; Noufi, Rommel] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Hsu, Wan-Ching] Univ Calif Los Angeles, Dept Mat Sci & Engn, Los Angeles, CA 90095 USA. RP Repins, IL (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM ingrid.repins@nrel.gov; manuel.romero@nrel.gov; jian.li@nrel.gov; Suhuai.Wei@nrel.gov; darius.kuciauskas@nrel.gov; chun.sheng.jiang@nrel.gov; Carolyn.Beall@nrel.gov; Clay.DeHart@nrel.gov; jonathan.mann@nrel.gov; ching.hsu@ucla.edu; glenn.teeter@nrel.gov; Alan.Goodrich@nrel.gov; Rommel.Noufi@nrel.gov RI jiang, chun-sheng/F-7839-2012; Li, Jian/B-1627-2016 FU Alliance for Sustainable Energy, LLC [DE-AC36-08GO28308]; U.S. Department of Energy; California NanoSystem Institute FX Manuscript received May 14, 2012; revised August 21, 2012; accepted August 22, 2012. Date of publication September 19, 2012; date of current version December 19, 2012. This work was supported by the Alliance for Sustainable Energy, LLC, under Contract DE-AC36-08GO28308 along with the U.S. Department of Energy. (The Alliance for Sustainable Energy, LLC, is the manager and operator of the National Renewable Energy Laboratory.) The work of W.-C. Hsu was supported by the California NanoSystem Institute. NR 52 TC 31 Z9 31 U1 3 U2 82 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 2156-3381 J9 IEEE J PHOTOVOLT JI IEEE J. Photovolt. PD JAN PY 2013 VL 3 IS 1 BP 439 EP 445 DI 10.1109/JPHOTOV.2012.2215842 PG 7 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA 137KF UT WOS:000318434000068 ER PT J AU Mann, JR Kempe, M Repins, I Duda, A Glick, S Kanevce, A AF Mann, J. R. Kempe, M. Repins, I. Duda, A. Glick, S. Kanevce, A. TI A Dry Heat-Induced Effect of Using Silver in CIGS Gridlines SO IEEE JOURNAL OF PHOTOVOLTAICS LA English DT Article DE Buffer; Cu(In,Ga)Se-2 (CIGS); diffusion; gridlines; photocurrent; silver ID FILM SOLAR-CELLS AB The ease with which screen-printed silver is deposited and its high conductivity make it an appealing choice for gridline material on CIGS-based photovoltaic devices. However, present results suggest silver diffusion into the device can cause severe reductions in efficiency after as little as 200 h at 85 degrees C. Dramatic reductions in fill factor, characterized by unusual inflections in the power quadrant of current-voltage curves, are observed for devices with silver gridlines but not for those with nickel or aluminum gridlines. The shape of the current-voltage curves demonstrate that the degradation mode is not simply due to changes in resistance but is consistent with the creation of a secondary barrier near the device junction. C1 [Mann, J. R.; Kempe, M.; Repins, I.; Duda, A.; Glick, S.; Kanevce, A.] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Mann, JR (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM jonathan.mann@nrel.gov; Michael.Kempe@NREL.gov; ingrid.repins@nrel.gov; anna.duda@nrel.gov; Stephen.Glick@NREL.GOV; Ana.Kanevce@nrel.gov FU U.S. Department of Energy [DE-AC36-08-GO28308]; National Renewable Energy Laboratory FX Manuscript received March 7, 2012; revised September 14, 2012; accepted September 14, 2012. Date of publication October 24, 2012; date of current version December 19, 2012. This work was supported by the U.S. Department of Energy under Contract DE-AC36-08-GO28308 with the National Renewable Energy Laboratory. NR 13 TC 0 Z9 0 U1 1 U2 13 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 2156-3381 J9 IEEE J PHOTOVOLT JI IEEE J. Photovolt. PD JAN PY 2013 VL 3 IS 1 BP 457 EP 460 DI 10.1109/JPHOTOV.2012.2219852 PG 4 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA 137KF UT WOS:000318434000071 ER PT J AU Mann, J Li, J Repins, I Ramanathan, K Glynn, S DeHart, C Noufi, R AF Mann, Jonathan Li, Jian Repins, Ingrid Ramanathan, Kannan Glynn, Stephen DeHart, Clay Noufi, Rommel TI Reflection Optimization for Alternative Thin-Film Photovoltaics SO IEEE JOURNAL OF PHOTOVOLTAICS LA English DT Article DE Cadmium sulfide (CdS); copper indium gallium selenide (CIGS); copper zinc tin selenide (CZTS); reflection; zinc sulfide (ZnS) ID SOLAR-CELLS; SINGLE-LAYER; EFFICIENCY AB The recent improvements in efficiencies for kesterite (copper zinc tin selenide, CZTS) devices warrant an investigation into how the kesterite device stack can best be capped to minimize losses due to reflection. Additionally, ongoing efforts to replace the cadmium sulfide (CdS) layer in copper indium gallium selenide (CIGS)-based devices, most notably with zinc sulfide (ZnS), need to be accompanied by a similar investigation into how to best finish a CIGS/ZnS stack to minimize reflection losses. An optical analysis of how CZTS/CdS and CIGS/ZnS devices reflect light has been performed for the purpose of optimizing the transparent conducting oxide and antireflection layers for each stack. This research addresses what is similar and what is different between the alternative stacks and the routine CIGS/CdS stack and how to best reduce the reflection losses for each situation. C1 [Mann, Jonathan; Li, Jian; Repins, Ingrid; Ramanathan, Kannan; Glynn, Stephen; DeHart, Clay; Noufi, Rommel] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Li, Jian] Colorado Sch Mines, Dept Phys, Golden, CO 80401 USA. RP Mann, J (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM jonathan.mann@nrel.gov; Jian2.Li@nrel.gov; ingrid.repins@nrel.gov; kannan.ramanathan@nrel.gov; Stephen.Glynn@nrel.gov; Clay.DeHart@nrel.gov; Rommel.Noufi@nrel.gov FU U.S Department of Energy [DE-AC36-08GO28308]; National Renewable Energy Laboratory FX Manuscript received May 18, 2012; accepted September 26, 2012. Date of publication November 12, 2012; date of current version December 19, 2012. This work was supported by the U.S Department of Energy under Contract DE-AC36-08GO28308 with the National Renewable Energy Laboratory. NR 14 TC 8 Z9 8 U1 1 U2 49 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 2156-3381 J9 IEEE J PHOTOVOLT JI IEEE J. Photovolt. PD JAN PY 2013 VL 3 IS 1 BP 472 EP 475 DI 10.1109/JPHOTOV.2012.2224321 PG 4 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA 137KF UT WOS:000318434000074 ER PT J AU Ishizuka, S Mansfield, LM DeHart, C Scott, M To, B Young, MR Egaas, B Noufi, R AF Ishizuka, Shogo Mansfield, Lorelle M. DeHart, Clay Scott, Marty To, Bobby Young, Matthew R. Egaas, Brian Noufi, Rommel TI Rapid Fabrication of Cu(In,Ga)Se-2 Thin Films by the Two-Step Selenization Process SO IEEE JOURNAL OF PHOTOVOLTAICS LA English DT Article DE Copper indium gallium diselenide; Cu(In,Ga)Se-2 (CIGS); photovoltaic cells; selenization; thin films ID SOLAR-CELLS; SE-VAPOR; PRECURSORS; CUINSE2; PHASE AB Two-step processes currently used for the industrial Cu(In,Ga)Se-2 (CIGS) module production require a long process time of several hours for the CIGS absorber formation. In this paper, we are studying the reaction pathway to rapid selenization of stacked metal precursors in elemental Se vapor. The objective is to understand the reaction kinetics to find the best precursor structure and the optimal selenization conditions to form high-quality CIGS films with proper Ga depth profiles. In addition to stacked metal precursors, the effect of the use of Se-containing precursors was also examined. As expected, the stacking order of the metal precursors influences the properties of the resulting CIGS absorbers. The Cu amount deposited for the precursor formation critically affected the final film and cell properties, as well. We also found that the formation of CIGS films with large grain sizes and flat Ga depth profiles was possible even for [Cu]/([In] + [Ga]) < 1 conditions with the use of particular precursor structures and selenization conditions. The results suggest that the selenization reaction pathway can be dictated with the precursor structure, and further improvements are expected by controlling reaction kinetics with precursor structure modification. C1 [Ishizuka, Shogo; Mansfield, Lorelle M.; DeHart, Clay; Scott, Marty; To, Bobby; Young, Matthew R.; Egaas, Brian; Noufi, Rommel] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Ishizuka, Shogo] Natl Inst Adv Ind Sci & Technol, Tsukuba, Ibaraki 3058568, Japan. RP Ishizuka, S (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM shogo-ishizuka@aist.go.jp; lorelle.mansfield@nrel.gov; clay.dehart@nrel.gov; marty.scott@nrel.gov; bobby.to@nrel.gov; matthew.young@nrel.gov; brian.egaas@nrel.gov; rommel.noufi@nrel.gov FU U.S. Department of Energy SunShot Program's Funding of the National Renewable Energy Laboratory Core Science and Technology Activities; Foundational Program for Advancing Conversion Efficiency FX Manuscript received May 21, 2012; revised August 27, 2012 and September 21, 2012; accepted September 27, 2012. Date of publication November 12, 2012; date of current version December 19, 2012. This work was supported by the U.S. Department of Energy SunShot Program's Funding of the National Renewable Energy Laboratory Core Science and Technology Activities, and Foundational Program for Advancing Conversion Efficiency. NR 14 TC 5 Z9 5 U1 2 U2 38 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 2156-3381 J9 IEEE J PHOTOVOLT JI IEEE J. Photovolt. PD JAN PY 2013 VL 3 IS 1 BP 476 EP 482 DI 10.1109/JPHOTOV.2012.2222868 PG 7 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA 137KF UT WOS:000318434000075 ER PT S AU Hao, Q AF Hao, Qiu CA STAR Collaboration GP IOP TI Heavy Flavor Results from STAR SO INTERNATIONAL CONFERENCE ON HEAVY ION COLLISIONS IN THE LHC ERA SE Journal of Physics Conference Series LA English DT Proceedings Paper CT International Conference on Heavy Ion Collisions in the LHC Era CY JUL 16-20, 2012 CL Quy Nhon, VIETNAM SP European Res Council, Xunta Galicia, EMMI, Agence Nationale Rech, Lab Annecy-le-Vieux Physique Theorique ID COLLISIONS AB Heavy flavor quarks are considered to be unique probes of the medium created in high energy heavy ion collisions. These proceedings report selected STAR results from various measurements of heavy flavor production, including J/psi, suppression and collectivity, Upsilon suppression, ratio of bottom-decay electrons to charm-decay electrons, D meson spectra and charm cross section. C1 [Hao, Qiu; STAR Collaboration] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Hao, Q (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM hqiu@lbl.gov NR 20 TC 0 Z9 0 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA DIRAC HOUSE, TEMPLE BACK, BRISTOL BS1 6BE, ENGLAND SN 1742-6588 J9 J PHYS CONF SER PY 2013 VL 422 AR 012013 DI 10.1088/1742-6596/422/1/012013 PG 4 WC Physics, Nuclear SC Physics GA BEW61 UT WOS:000318416900013 ER PT J AU Kaur, N Zhao, QZ Xie, Q Hu, JP AF Kaur, Navneet Zhao, Qingzhen Xie, Qi Hu, Jianping TI Arabidopsis RING Peroxins are E3 Ubiquitin Ligases that Interact with Two Homologous Ubiquitin Receptor Proteins SO JOURNAL OF INTEGRATIVE PLANT BIOLOGY LA English DT Article DE Arabidopsis; RING domain proteins; peroxisomes; ubiquitin receptor ID PEROXISOMAL IMPORT RECEPTOR; U-BOX; PLANT PEROXISOMES; PEX5P; BIOGENESIS; FINGER; FAMILY; PROTEASOME; THALIANA; DOMAIN AB Peroxisomes are essential eukaryotic organelles that mediate various metabolic processes. Peroxisome import depends on a group of peroxisome biogenesis factors called peroxins, many of which are evolutionarily conserved. PEX2, PEX10, and PEX12 are three RING-finger-domain-containing integral membrane peroxins crucial for protein import. In yeast (Saccharomyces cerevisae), RING peroxins act as E3 ligases, facilitating the recycling of the peroxisome import receptor protein PEX5 through ubiquitination. In plants, RING peroxins are essential to plant vitality. To elucidate the mode of action of the plant RING peroxins, we employed in vitro assays to show that the Arabidopsis RING peroxins also have E3 ligase activities. We also identified a PEX2-interacting protein, DSK2b, which is a member of the ubiquitin receptor family known to function as shuttle factors ferrying polyubiquitinated substrates to the proteasome for degradation. DSK2b and its tandem duplicate DSK2a are localized in the cytosol and the nucleus, and both interact with the RING domain of PEX2 and PEX12. DSK2 artificial microRNA lines did not display obvious defects in plant growth or peroxisomal processes, indicating functional redundancies among Arabidopsis ubiquitin receptor proteins. Our results suggest that Arabidopsis RING peroxins can function as E3 ligases and act together with the ubiquitin receptor protein DSK2 in the peroxisomal membrane-associated protein degradation system. C1 [Kaur, Navneet; Hu, Jianping] Michigan State Univ, MSU DOE Plant Res Lab, E Lansing, MI 48824 USA. [Zhao, Qingzhen; Xie, Qi] Chinese Acad Sci, Inst Genet & Dev Biol, Beijing 100101, Peoples R China. RP Hu, JP (reprint author), Michigan State Univ, MSU DOE Plant Res Lab, E Lansing, MI 48824 USA. EM huji@msu.edu FU National Science Foundation [MCB 0618335]; Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Sciences, Office of Science, US Department of Energy [DE-FG02-91ER20021] FX The authors would like to thank the Arabidopsis Biological Resource Center (ABRC) for providing seeds of the DSK2 T-DNA insertion mutants, and Jilian Fan for genotyping the mutants, Judy Callis (University of California, Davis) for the UBC8 and CIP8 constructs, Sheng Yang He (Michigan State University) for the modified pB42AD plasmid, and Detlef Weigel (Max Planck Institute for Developmental Biology, Tubingen, Germany) for sharing the amiRNA backbone pRS300 vector. This work was supported by grants from the National Science Foundation Arabidopsis 2010 program (MCB 0618335) and the Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Sciences, Office of Science, US Department of Energy (DE-FG02-91ER20021) to J. H. NR 61 TC 20 Z9 26 U1 2 U2 12 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1672-9072 J9 J INTEGR PLANT BIOL JI J. Integr. Plant Biol. PD JAN PY 2013 VL 55 IS 1 SI SI BP 108 EP + DI 10.1111/jipb.12014 PG 13 WC Biochemistry & Molecular Biology; Plant Sciences SC Biochemistry & Molecular Biology; Plant Sciences GA 139RA UT WOS:000318600300001 PM 23336935 ER PT J AU El-Hachemi, Z Escudero, C Acosta-Reyes, F Casas, MT Altoe, V Aloni, S Oncins, G Sorrenti, A Crusats, J Campos, JL Ribo, JM AF El-Hachemi, Zoubir Escudero, Carlos Acosta-Reyes, Francisco Teresa Casas, M. Altoe, Virginia Aloni, Shaul Oncins, Gerard Sorrenti, Alessandro Crusats, Joaquim Lourdes Campos, J. Ribo, Josep M. TI Structure vs. properties - chirality, optics and shapes - in amphiphilic porphyrin J-aggregates SO JOURNAL OF MATERIALS CHEMISTRY C LA English DT Article ID SUPRAMOLECULAR CHIRALITY; SYMMETRY-BREAKING; STIRRED SOLUTIONS; AQUEOUS-SOLUTION; WATER; SPECTRA; DYE; CRYSTALLIZATION; ASSEMBLIES; MICROSCOPY AB The structure of the meso-tetrakis(4-sulfonatophenyl) porphyrin (TPPS4) J-aggregates could be determined by X-ray and electron diffraction methods. A sheet-like architecture reveals the relationship between structure and chirality, optics and shapes of the J-aggregates of the meso 4-sulfonatophenyl- and phenyl-substituted porphyrins. The structure of the J-aggregates of H4TPPS4 belongs to the chiral space group P2(1) and includes four porphyrin molecules in its unit cell. The intermolecular stabilization of the zwitterionic units by hydrogen bonding and electrostatic interactions between the positively charged central NH groups and the periphery anionic sulfonato groups results in a structure of porphyrins sheets along the [(1) over bar 01] plane direction. The structure of the sheet on the [(1) over bar 01] plane is already chiral and its molecular architecture explains the simultaneous presence of H- and J-aggregate bands in their absorption spectra. This structure also accounts for the high similarity observed between the absorption spectra of different mesomorphs of the same substance and even between different members of the series of meso-4-sulfonatophenyl- and aryl-substituted diprotonated porphyrins. The possibility, or not, of the sheet-like structure on [(1) over bar 01] to interact with other layers, either through ionic or hydrophobic interactions, depends on the substitution pattern at the meso-positions of the porphyrin ring. Thus, the different morphologies of the particles [mono- bi- and multilayered] of this series of J-aggregates are explained taking into account the role that the fourth meso-substituent plays in the interlayer stabilization. The results suggest that supramolecular helicity, previously detected in several J-aggregates, is not the explanation of their chirality but would be the expression of the intrinsic chirality of the packing between building blocks. C1 [El-Hachemi, Zoubir; Sorrenti, Alessandro; Crusats, Joaquim; Ribo, Josep M.] Univ Barcelona IECC UB, Inst Cosmos Sci, Dept Organ Chem, Barcelona 08028, Catalonia, Spain. [Escudero, Carlos] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Acosta-Reyes, Francisco; Teresa Casas, M.; Lourdes Campos, J.] UPC, Dept Chem Engn, Barcelona 08028, Catalonia, Spain. [Altoe, Virginia; Aloni, Shaul] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Oncins, Gerard] Univ Barcelona, Nanometr Tech Unit Sci & Technol Serv CCiTUB, E-08028 Barcelona, Catalonia, Spain. RP El-Hachemi, Z (reprint author), Univ Barcelona IECC UB, Inst Cosmos Sci, Dept Organ Chem, C Marti & Franques 1, Barcelona 08028, Catalonia, Spain. EM jmribo@ub.edu RI Sorrenti, Alessandro/J-9442-2014; Campos, J.Lourdes/N-7336-2014; Foundry, Molecular/G-9968-2014; Campos, Juan/N-1211-2014; Escudero, Carlos/F-8044-2011; OI Campos, J.Lourdes/0000-0002-4136-7082; Campos, Juan/0000-0002-2479-4373; Escudero, Carlos/0000-0001-8716-9391; Casas Becerra, Maria Teresa/0000-0002-5309-8246 NR 57 TC 34 Z9 34 U1 2 U2 56 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2050-7526 J9 J MATER CHEM C JI J. Mater. Chem. C PY 2013 VL 1 IS 20 BP 3337 EP 3346 DI 10.1039/c3tc30299g PG 10 WC Materials Science, Multidisciplinary; Physics, Applied SC Materials Science; Physics GA 136KQ UT WOS:000318361200009 ER PT J AU Johnson, JL Dalla Vecchia, C Khochfar, S AF Johnson, Jarrett L. Dalla Vecchia, Claudio Khochfar, Sadegh TI The First Billion Years project: the impact of stellar radiation on the co-evolution of Populations II and III SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE molecular processes; galaxies: formation; galaxies: high-redshift; intergalactic medium; cosmology: theory; early Universe ID SUPERMASSIVE BLACK-HOLES; PAIR-INSTABILITY SUPERNOVAE; INITIAL MASS FUNCTION; HIGH-REDSHIFT PROTOGALAXIES; STAR-FORMATION HISTORY; LAMBDA-CDM UNIVERSE; DARK-MATTER HALOES; METAL-FREE STARS; CHEMICAL ENRICHMENT; PRIMORDIAL STARS AB With the first metal enrichment by Population III (Pop III) supernovae (SNe), the formation of the first metal-enriched, Pop II stars becomes possible. In turn, Pop III star formation and early metal enrichment are slowed by the high-energy radiation emitted by Pop II stars. Thus, through the SNe and radiation they produce, Pops II and III co-evolve in the early Universe, one regulated by the other. We present large (4 Mpc)(3), high-resolution cosmological simulations in which we self-consistently model early metal enrichment and the stellar radiation responsible for the destruction of the coolants (H-2 and HD) required for Pop III star formation. We find that the molecule-dissociating stellar radiation produced both locally and over cosmological distances reduces the Pop III star formation rate at z greater than or similar to 10 by up to an order of magnitude, to a rate per comoving volume of less than or similar to 10(-4) M-circle dot yr(-1) Mpc(-3), compared to the case in which this radiation is not included. However, we find that the effect of Lyman-Werner (LW) feedback is to enhance the amount of Pop II star formation. We attribute this to the reduced rate at which gas is blown out of dark matter haloes by SNe in the simulation with LW feedback, which results in larger reservoirs for metal-enriched star formation. Even accounting for metal enrichment, molecule-dissociating radiation and the strong suppression of low-mass galaxy formation due to reionization at z less than or similar to 10, we find that Pop III stars are still formed at a rate of similar to 10(-5) M-circle dot yr(-1) Mpc(-3) down to z similar to 6. This suggests that the majority of primordial pair-instability SNe that may be uncovered in future surveys will be found at z less than or similar to 10. We also find that the molecule-dissociating radiation emitted from Pop II stars may destroy H-2 molecules at a high enough rate to suppress gas cooling and allow for the formation of supermassive primordial stars which collapse to form similar to 10(5) M-circle dot black holes. C1 [Johnson, Jarrett L.] Los Alamos Natl Lab, Nucl & Particle Phys Astrophys & Cosmol Grp T2, Los Alamos, NM 87545 USA. [Johnson, Jarrett L.; Dalla Vecchia, Claudio; Khochfar, Sadegh] Max Planck Inst Extraterr Phys, Theoret Modeling Cosm Struct Grp, D-85748 Garching, Germany. RP Johnson, JL (reprint author), Los Alamos Natl Lab, Nucl & Particle Phys Astrophys & Cosmol Grp T2, POB 1663, Los Alamos, NM 87545 USA. EM jlj@lanl.gov OI Dalla Vecchia, Claudio/0000-0002-2620-7056 FU US Department of Energy through the LANL/LDRD Program; Marie Curie Reintegration Grant [FP7-RG-256573] FX JLJ gratefully acknowledges the support of the US Department of Energy through the LANL/LDRD Program. CDV acknowledges support by Marie Curie Reintegration Grant FP7-RG-256573. We acknowledge helpful discussions with Bhaskar Agarwal, Volker Bromm, UmbertoMaio, Jan-Pieter Paardekooper and Dan Whalen, and we thank Andrew Davis for comments on an early draft. NR 136 TC 55 Z9 55 U1 1 U2 3 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD JAN PY 2013 VL 428 IS 3 BP 1857 EP 1872 DI 10.1093/mnras/sts011 PG 16 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 134RA UT WOS:000318230700001 ER PT J AU Zheng, HM AF Zheng, Haimei TI Using molecular tweezers to move and image nanoparticles SO NANOSCALE LA English DT Article ID NANOMETRIC OPTICAL TWEEZERS; ATOMIC-FORCE MICROSCOPE; METAL NANOPARTICLES; GOLD NANOPARTICLES; ELECTRON-BEAM; MANIPULATION; PARTICLES; TRAP; NANOMANIPULATION; NANOWIRES AB The ability to manipulate nanoparticles is significant in nanoscale science and technology. As sizes of the objects scale down to the sub-10 nm regime, it imposes a great challenge for the conventional optical tweezers. There has been much effort to explore alternative manipulation methods including using nanostructures, electron beams, scanning probes, etc. In this paper, an overview of the latest advances in trapping and manipulation of nanoparticles with a focus on the emergent electron tweezers is provided. C1 Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94708 USA. RP Zheng, HM (reprint author), Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94708 USA. EM hmzheng@lbl.gov FU US Department of Energy Office of Science Early Career Research Program FX HZ thanks the support of the US Department of Energy Office of Science Early Career Research Program. NR 59 TC 8 Z9 8 U1 2 U2 55 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2040-3364 EI 2040-3372 J9 NANOSCALE JI Nanoscale PY 2013 VL 5 IS 10 BP 4070 EP 4078 DI 10.1039/c3nr00737e PG 9 WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 136LC UT WOS:000318362400004 PM 23592008 ER PT J AU Wang, GM Ling, YC Lu, XH Zhai, T Qian, F Tong, YX Li, Y AF Wang, Gongming Ling, Yichuan Lu, Xihong Zhai, Teng Qian, Fang Tong, Yexiang Li, Yat TI A mechanistic study into the catalytic effect of Ni(OH)(2) on hematite for photoelectrochemical water oxidation SO NANOSCALE LA English DT Article ID NICKEL-OXIDE; NANOWIRE ARRAYS; OXYGEN; PHOTOANODES; ELECTRODES; CO; NANOSTRUCTURES; PHOTOOXIDATION; PERFORMANCE; CONVERSION AB We report a mechanistic study of the catalytic effect of Ni(OH)(2) on hematite nanowires for photoelectrochemical water oxidation. Ni compounds have been shown to be good catalysts for electrochemical and photoelectrochemical water oxidation. While we also observed improved photocurrents for Ni-catalyst decorated hematite photoanodes, we found that the photocurrents decay rapidly, indicating the photocurrents were not stable. Importantly, we revealed that the enhanced photocurrent was due to water oxidation as well as the photo-induced charging effect. In addition to oxidizing water, the photoexcited holes generated in hematite efficiently oxidize Ni2+ to Ni3+ (0.35 V vs. Ag/AgCl). The instability of photocurrent was due to the depletion of Ni2+. We proposed that the catalytic mechanism of the Ni(II) catalyst for water oxidation is a two-step process that involves the fast initial oxidation of Ni2+ to Ni3+, and followed by the slow oxidation of Ni3+ to Ni4+, which is believed to be the active catalytic species for water oxidation. The catalytic effect of the Ni(II) catalyst was limited by the slow formation of Ni4+. Finally, we elucidated the real catalytic performance of Ni(OH)(2) on hematite for photoelectrochemical water oxidation by suppressing the photoinduced charging effect. This work could provide important insights for future studies on Ni based catalyst modified photoelectrodes for water oxidation. C1 [Wang, Gongming; Ling, Yichuan; Lu, Xihong; Zhai, Teng; Tong, Yexiang; Li, Yat] Univ Calif Santa Cruz, Dept Chem & Biochem, Santa Cruz, CA 95064 USA. [Lu, Xihong; Zhai, Teng; Tong, Yexiang] SunYat Sen Univ, Sch Chem & Chem Engn, KLGHEI Environm & Energy Chem, MOE,Key Lab Bioinorgan & Synthet Chem, Guangzhou 510275, Guangdong, Peoples R China. [Qian, Fang] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94550 USA. RP Li, Y (reprint author), Univ Calif Santa Cruz, Dept Chem & Biochem, Santa Cruz, CA 95064 USA. EM yli@chemistry.ucsc.edu RI Wang, Gongming/C-4555-2012; Lu, Xihong/L-5171-2015; Ling, Yichuan/I-9567-2016; OI Lu, Xihong/0000-0002-6764-0024; Li, Yat/0000-0002-8058-2084 FU United States NSF [DMR-0847786]; Natural Science Foundations of China [90923008, J1103305]; Natural Science Foundations of Guangdong Province [9251027501000002]; University of California, Santa Cruz; Academic New Artist Ministry of Education Doctoral Post Graduate (China); China Scholarship Council FX Y.L. acknowledges the financial support from United States NSF (DMR-0847786). Y.X.T. acknowledges the financial support from the Natural Science Foundations of China (90923008 and J1103305) and the Natural Science Foundations of Guangdong Province (9251027501000002). G.M.W. acknowledges the financial support of Chancellor's Dissertation Year Fellowship at the University of California, Santa Cruz. X. H. L. thanks the Academic New Artist Ministry of Education Doctoral Post Graduate (China) and China Scholarship Council for financial support. NR 35 TC 52 Z9 52 U1 8 U2 109 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2040-3364 J9 NANOSCALE JI Nanoscale PY 2013 VL 5 IS 10 BP 4129 EP 4133 DI 10.1039/c3nr00569k PG 5 WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 136LC UT WOS:000318362400012 PM 23563928 ER PT J AU Wieser, ME Holden, N Coplen, TB Bohlke, JK Berglund, M Brand, WA De Bievre, P Groning, M Loss, RD Meija, J Hirata, T Prohaska, T Schoenberg, R O'Connor, G Walczyk, T Yoneda, S Zhu, XK AF Wieser, Michael E. Holden, Norman Coplen, Tyler B. Boehlke, John K. Berglund, Michael Brand, Willi A. De Bievre, Paul Groening, Manfred Loss, Robert D. Meija, Juris Hirata, Takafumi Prohaska, Thomas Schoenberg, Ronny O'Connor, Glenda Walczyk, Thomas Yoneda, Shige Zhu, Xiang-Kun TI Atomic weights of the elements 2011 (IUPAC Technical Report) SO PURE AND APPLIED CHEMISTRY LA English DT Article DE atomic-weight intervals; atomic-weight ranges; bromine; conventional atomic-weight values; germanium; half-lives; indium; IUPAC Inorganic Chemistry Division; magnesium; mercury; standard atomic weights ID PLASMA-MASS SPECTROMETRY; ISOTOPIC COMPOSITION; MAGNESIUM; RATIOS; REFERENCES; GRAPHS; TABLES AB The biennial review of atomic-weight determinations and other cognate data has resulted in changes for the standard atomic weights of five elements. The atomic weight of bromine has changed from 79.904(1) to the interval [79.901, 79.907], germanium from 72.63(1) to 72.630(8), indium from 114.818(3) to 114.818(1), magnesium from 24.3050(6) to the interval [24.304, 24.307], and mercury from 200.59(2) to 200.592(3). For bromine and magnesium, assignment of intervals for the new standard atomic weights reflects the common occurrence of variations in the atomic weights of those elements in normal terrestrial materials. C1 [Wieser, Michael E.] Univ Calgary, Dept Phys & Astron, Calgary, AB T2N 1N4, Canada. [Holden, Norman] Brookhaven Natl Lab, Upton, NY 11973 USA. [Coplen, Tyler B.; Boehlke, John K.] US Geol Survey, Reston, VA 22092 USA. [Berglund, Michael] Inst Reference Mat & Measurements, Geel, Belgium. [Brand, Willi A.] Max Planck Inst Biogeochem, D-07745 Jena, Germany. [Groening, Manfred] IAEA, Seibersdorf, Austria. [Loss, Robert D.] Curtin Univ Technol, Dept Appl Phys, Perth, WA, Australia. [Meija, Juris] Natl Res Council Canada, Ottawa, ON, Canada. [Hirata, Takafumi] Kyoto Univ, Kyoto, Japan. [Prohaska, Thomas] Univ Nat Resources & Appl Life Sci, Dept Chem, Vienna, Austria. [Schoenberg, Ronny] Univ Tubingen, Inst Geosci, Tubingen, Germany. [O'Connor, Glenda] New Brunswick Lab, Argonne, IL USA. [Walczyk, Thomas] Natl Univ Singapore, Dept Chem Sci, Singapore 117548, Singapore. [Walczyk, Thomas] Natl Univ Singapore, Dept Biochem Med, Singapore 117548, Singapore. [Yoneda, Shige] Natl Museum Nat & Sci, Tokyo, Japan. [Zhu, Xiang-Kun] Chinese Acad Geol Sci, Beijing, Peoples R China. RP Wieser, ME (reprint author), Univ Calgary, Dept Phys & Astron, Calgary, AB T2N 1N4, Canada. EM mwieser@ucalgary.ca RI Brand, Willi/D-2043-2009; OI Meija, Juris/0000-0002-3349-5535 FU IUPAC Inorganic Chemistry Division, Commission on Isotopic Abundances and Atomic Weights; U.S. Geological Survey National Research Program; IUPAC projects [2007-029-1-200, 2007-028-1-200, 2007-038-3-200, 2009-025-2-200, 2009-029-1-200] FX Sponsoring body: IUPAC Inorganic Chemistry Division, Commission on Isotopic Abundances and Atomic Weights: see more details on p. 1076.; The support of the U.S. Geological Survey National Research Program made this report possible. The following IUPAC projects contributed to this Technical Report: 2007-029-1-200, 2007-028-1-200, 2007-038-3-200, 2009-025-2-200, and 2009-029-1-200. NR 51 TC 157 Z9 157 U1 7 U2 68 PU INT UNION PURE APPLIED CHEMISTRY PI RES TRIANGLE PK PA 104 TW ALEXANDER DR, PO BOX 13757, RES TRIANGLE PK, NC 27709-3757 USA SN 0033-4545 J9 PURE APPL CHEM JI Pure Appl. Chem. PY 2013 VL 85 IS 5 BP 1047 EP 1078 DI 10.1351/PAC-REP-13-03-02 PG 32 WC Chemistry, Multidisciplinary SC Chemistry GA 137AY UT WOS:000318408300009 ER PT S AU Huang, K Heinrich, H Keiser, DD Sohn, YH AF Huang, K. Heinrich, H. Keiser, D. D., Jr. Sohn, Y. H. BE Ochsner, A Belova, I Murch, G TI Fuel-Matrix Chemical Interaction Between U-7wt.%Mo Alloy and Mg SO RECENT ADVANCES IN MASS TRANSPORT IN ENGINEERING MATERIALS SE Defect and Diffusion Forum LA English DT Article; Book Chapter DE U-Mo alloy; Mg; interdiffusion; diffusion barrier ID MO DISPERSION FUEL; HIGH-DENSITY; AL; INTERDIFFUSION AB A solid-to-solid, U-7wt.%Mo vs. Mg diffusion couple was assembled and annealed at 550 degrees C for 96 hours. The microstructure in the interdiffusion zone and the development of concentration profiles were examined via scanning electron microscopy, transmission electron microscopy(TEM) and X-ray energy dispersive spectroscopy. A TEM specimen was prepared at the interface between U-7wt.%Mo and Mg using focused ion beam in-situ lift-out. The U-7wt.%Mo alloy was bonded well to the Mg at the atomic scale, without any evidence of oxidation, cracks or pores. Despite the good bonding, very little or negligible interdiffusion was observed. This is consistent with the expectation based on negligible solubilities according to the equilibrium phase diagrams. Along with other desirable properties, Mg is a potential inert matrix or barrier material for U-Mo fuel alloy system being developed for the Reduced Enrichment for Research and Test Reactor (RERTR) program. C1 [Huang, K.; Sohn, Y. H.] Univ Cent Florida, Dept Mech Mat & Aerosp Engn, Adv Mat Proc & Anal Ctr, Orlando, FL 32816 USA. [Heinrich, H.] Univ Cent Florida, Dept Phys, Orlando, FL 32816 USA. [Keiser, D. D., Jr.] Idaho Natl Lab, Nucl Fuels & Mat Div, Idaho Falls, ID 83415 USA. RP Huang, K (reprint author), Univ Cent Florida, Dept Mech Mat & Aerosp Engn, Adv Mat Proc & Anal Ctr, Orlando, FL 32816 USA. EM Yongho.Sohn@ucf.edu NR 21 TC 5 Z9 5 U1 1 U2 2 PU TRANS TECH PUBLICATIONS LTD PI STAFA-ZURICH PA LAUBLSRUTISTR 24, CH-8717 STAFA-ZURICH, SWITZERLAND SN 1012-0386 J9 DEFECT DIFFUS FORUM PY 2013 VL 333 BP 199 EP 206 DI 10.4028/www.scientific.net/DDF.333.199 PG 8 WC Materials Science, Multidisciplinary; Transportation Science & Technology SC Materials Science; Transportation GA BEN26 UT WOS:000317436200018 ER PT J AU Mohanty, D Kalnaus, S Meisner, RA Safat, AS Li, JL Payzant, EA Rhodes, K Wood, DL Daniel, C AF Mohanty, Debasish Kalnaus, Sergiy Meisner, Roberta A. Safat, Athena S. Li, Jianlin Payzant, E. Andrew Rhodes, Kevin Wood, David L., III Daniel, Claus TI Structural transformation in a Li1.2Co0.1Mn0.55Ni0.15O2 lithium-ion battery cathode during high-voltage hold SO RSC ADVANCES LA English DT Article ID POSITIVE-ELECTRODE MATERIALS; X-RAY-DIFFRACTION; OXIDES; STABILITY; EVOLUTION; CAPACITY AB A decrease in the c-lattice parameter was observed in Li1.2Co0.1Mn0.55Ni0.15O2 during constant voltage holding at 4.5 V by in situ X-ray diffraction. Comparison of magnetic susceptibility data before and after high-voltage hold reveals the change in average oxidation states of transition metal ions during high-voltage holding process. Transmission electron microscopy studies show the spinel reflections with fundamental trigonal spots from the particles after high-voltage hold indicating substantial structural modification. The structural transformation was believed to occur due to the oxygen release and/or the migration of transition metal cations to lithium layer during constant voltage holding. C1 [Mohanty, Debasish; Kalnaus, Sergiy; Meisner, Roberta A.; Safat, Athena S.; Wood, David L., III] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37931 USA. [Li, Jianlin; Daniel, Claus] Oak Ridge Natl Lab, Energy & Transportat Sci Div, Oak Ridge, TN 37831 USA. [Payzant, E. Andrew] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. [Rhodes, Kevin] Ford Motor Co, Ford Res & Innovat Ctr, Dearborn, MI 48121 USA. [Daniel, Claus] Univ Tennessee, Bredesen Ctr Interdisciplinary Res & Grad Educ, Knoxville, TN 37996 USA. RP Mohanty, D (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37931 USA. EM mohantyd@ornl.gov; kalnauss@ornl.gov RI Payzant, Edward/B-5449-2009; Mohanty, Debasish/B-6207-2012; Daniel, Claus/A-2060-2008; Li, Jianlin/D-3476-2011 OI Payzant, Edward/0000-0002-3447-2060; Mohanty, Debasish/0000-0003-1141-0657; Daniel, Claus/0000-0002-0571-6054; Li, Jianlin/0000-0002-8710-9847 FU U.S. Department of Energy (DOE) [DE-AC05-00OR22725]; Office of Energy Efficiency and Renewable Energy for the Vehicle Technologies Office's Applied Battery Research Program; DOE, Basic Energy Sciences, Materials Sciences and Engineering Division; ORNL's ShaRE User Facility; Scientific User Facilities Division, Office of Basic Energy Sciences, DOE; DOE Vehicle Technologies Office (VTO) within Applied Battery Research (ABR) FX This research at Oak Ridge National Laboratory, managed by UT Battelle, LLC, for the U.S. Department of Energy (DOE) under contract DE-AC05-00OR22725, was sponsored by the Office of Energy Efficiency and Renewable Energy for the Vehicle Technologies Office's Applied Battery Research Program (Program Managers: Peter Faguy and David Howell). Part of this research was supported by the DOE, Basic Energy Sciences, Materials Sciences and Engineering Division and by ORNL's ShaRE User Facility, which is sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, DOE. The electrodes were produced at the DOE's Cell Fabrication Facility, Argonne National Laboratory, by Andrew Jansen and Bryant Polzin. The Cell Fabrication Facility is fully supported by the DOE Vehicle Technologies Office (VTO) within the core funding of the Applied Battery Research (ABR). The authors thank Dr. Daniel Abraham at Argonne National Laboratory for useful discussion. NR 31 TC 22 Z9 22 U1 7 U2 39 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2046-2069 J9 RSC ADV JI RSC Adv. PY 2013 VL 3 IS 20 BP 7479 EP 7485 DI 10.1039/c3ra40510a PG 7 WC Chemistry, Multidisciplinary SC Chemistry GA 135QF UT WOS:000318302900046 ER PT J AU Somma, RD Boixo, S AF Somma, R. D. Boixo, S. TI SPECTRAL GAP AMPLIFICATION SO SIAM JOURNAL ON COMPUTING LA English DT Article DE quantum algorithms; adiabatic quantum computing; quantum Monte-Carlo ID SIMULATING SPARSE HAMILTONIANS; QUANTUM COMPUTATION; ALGORITHMS; COMPLEXITY AB Many problems can be solved by preparing a specific eigenstate of some Hamiltonian H. The generic cost of quantum algorithms for these problems is determined by the inverse spectral gap of H for that eigenstate and the cost of evolving with H for some fixed time. The goal of spectral gap amplification is to construct a Hamiltonian H' with the same eigenstate as H but a bigger spectral gap, requiring that constant-time evolutions with H' and H are implemented with nearly the same cost. We show that a quadratic spectral gap amplification is possible when H satisfies a frustration-free property and give H' for these cases. This results in quantum speedups for optimization problems. It also yields improved constructions for adiabatic simulations of quantum circuits and for the preparation of projected entangled pair states, which play an important role in quantum many-body physics. Defining a suitable black-box model, we establish that the quadratic amplification is optimal for frustration-free Hamiltonians and that no spectral gap amplification is possible, in general, if the frustration-free property is removed. A corollary is that finding a similarity transformation between a stoquastic Hamiltonian and the corresponding stochastic matrix is hard in the black-box model, setting limits to the power of some classical methods that simulate quantum adiabatic evolutions. C1 [Somma, R. D.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Boixo, S.] Univ So Calif, Inst Informat Sci, Marina Del Rey, CA 90292 USA. RP Somma, RD (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM somma@lanl.gov; sboixo@isi.edu FU National Science Foundation through the CCF program; Laboratory Directed Research and Development Program at Los Alamos National Laboratory; Sandia National Laboratories; Lockheed Martin Corporation FX This author's work was supported by the National Science Foundation through the CCF program, and the Laboratory Directed Research and Development Program at Los Alamos National Laboratory and Sandia National Laboratories.; This author's work was partly supported by the Lockheed Martin Corporation. NR 44 TC 11 Z9 11 U1 0 U2 3 PU SIAM PUBLICATIONS PI PHILADELPHIA PA 3600 UNIV CITY SCIENCE CENTER, PHILADELPHIA, PA 19104-2688 USA SN 0097-5397 J9 SIAM J COMPUT JI SIAM J. Comput. PY 2013 VL 42 IS 2 BP 593 EP 610 DI 10.1137/120871997 PG 18 WC Computer Science, Theory & Methods; Mathematics, Applied SC Computer Science; Mathematics GA 136HU UT WOS:000318353800008 ER PT J AU Blass, T Romero, LA AF Blass, Timothy Romero, L. A. TI STABILITY OF ORDINARY DIFFERENTIAL EQUATIONS WITH COLORED NOISE FORCING SO SIAM JOURNAL ON CONTROL AND OPTIMIZATION LA English DT Article DE colored noise; parametric forcing; moment stability; Fokker-Planck operator; ladder operators ID FOKKER-PLANCK; OPERATORS AB We present a perturbation method for determining the moment stability of linear ordinary differential equations with parametric forcing by colored noise. In particular, the forcing arises from passing white noise through an nth order filter. We carry out a perturbation analysis based on a small parameter e that gives the amplitude of the forcing. Our perturbation analysis is based on a ladder operator approach to the vector Ornstein-Uhlenbeck process. We can carry out our perturbation expansion to any order in e, for a large class linear filters, and for quite arbitrary linear systems. As an example we apply our results to the stochastically forced Mathieu equation. C1 [Blass, Timothy] Carnegie Mellon Univ, Dept Math Sci, Pittsburgh, PA 15213 USA. [Romero, L. A.] Sandia Natl Labs, Computat Math & Algorithms Dept, Albuquerque, NM 87123 USA. RP Blass, T (reprint author), Carnegie Mellon Univ, Dept Math Sci, Pittsburgh, PA 15213 USA. EM tblass@andrew.cmu.edu; lromero@sandia.gov FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Computational Mathematics and Algorithms Department, Sandia National Laboratories, Albuquerque, NM 87123-1320 (lromero@sandia.gov). Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 25 TC 2 Z9 2 U1 0 U2 4 PU SIAM PUBLICATIONS PI PHILADELPHIA PA 3600 UNIV CITY SCIENCE CENTER, PHILADELPHIA, PA 19104-2688 USA SN 0363-0129 J9 SIAM J CONTROL OPTIM JI SIAM J. Control Optim. PY 2013 VL 51 IS 2 BP 1099 EP 1127 DI 10.1137/110855302 PG 29 WC Automation & Control Systems; Mathematics, Applied SC Automation & Control Systems; Mathematics GA 137AN UT WOS:000318406900012 ER PT S AU White, HB AF White, Herman B. BE Cunningham, BA TI Elementary Particle Physics at the Intensity Frontier SO WOMEN IN PHYSICS SE AIP Conference Proceedings LA English DT Meeting Abstract CT 4th IUPAP International Conference on Women in Physics CY APR 05-08, 2011 CL Stellenbosch, SOUTH AFRICA SP Int Union Pure & Appl Phys (IUPAP), Alfred P Sloan Fdn, Amer Assoc Advancement Sci, Amer Assoc Phys Teachers, Amer Phys Soc, Abdus Salam Int Centre Theoret Phys, Argonne Natl Lab, Deutsch Physikalische Gesell, Diverse Media Works LLC, Dorothy Jemison Fdn Excellence, Fermi Natl Accelerator Lab, Int Centre Theoret Phys, Japan Soc Appl Phys, Johns Hopkins Univ, John Wiley & Sons, Korean Phys Soc, LIGO-California Inst Technol, LOreal, Los Alamos Natl Lab, Massachusetts Inst Technol, Michigan State Univ, Natl Sci Council, Natl Inst Standards & Technol, Natl Sci Fdn, NE Univ, Coll Sci, Penn State Univ, Dept Phys, Phys Soc Japan, Scholast Inc, Stanford Univ, Thomas Jefferson Natl Accelerator Facil, UNESCO, Univ Dist Columbia, Univ Penn, Dept Phys & Astronomy, Dept Sci & Technol, Council Sci & Ind Res (Def Peace Safety & Secur; Mat Sci & Mfg; R&D; R&D Outcomes & Human Capital Dev), Juta Publishers, Natl Res Fdn, Nelson Mandela Metropolitan Univ, Dept Phys, S African Agcy Sci & Technol Awareness, S African Inst Phys, Square Kilometre Array Africa, Univ Pretoria, Dept Phys C1 [White, Herman B.] Fermilab Natl Accelerator Lab, Batavia, IL USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU AMER INST PHYSICS PI MELVILLE PA 2 HUNTINGTON QUADRANGLE, STE 1NO1, MELVILLE, NY 11747-4501 USA SN 0094-243X BN 978-0-7354-1138-8 J9 AIP CONF PROC PY 2013 VL 1517 BP 196 EP 196 PG 1 WC Physics, Applied SC Physics GA BEK11 UT WOS:000317018600111 ER PT S AU Seestrom, SJ AF Seestrom, Susan J. BE Cunningham, BA TI Measurement of the Beta Asymmetry in Neutron Decay Using Ultracold Neutrons SO WOMEN IN PHYSICS SE AIP Conference Proceedings LA English DT Meeting Abstract CT 4th IUPAP International Conference on Women in Physics CY APR 05-08, 2011 CL Stellenbosch, SOUTH AFRICA SP Int Union Pure & Appl Phys (IUPAP), Alfred P Sloan Fdn, Amer Assoc Advancement Sci, Amer Assoc Phys Teachers, Amer Phys Soc, Abdus Salam Int Centre Theoret Phys, Argonne Natl Lab, Deutsch Physikalische Gesell, Diverse Media Works LLC, Dorothy Jemison Fdn Excellence, Fermi Natl Accelerator Lab, Int Centre Theoret Phys, Japan Soc Appl Phys, Johns Hopkins Univ, John Wiley & Sons, Korean Phys Soc, LIGO-California Inst Technol, LOreal, Los Alamos Natl Lab, Massachusetts Inst Technol, Michigan State Univ, Natl Sci Council, Natl Inst Standards & Technol, Natl Sci Fdn, NE Univ, Coll Sci, Penn State Univ, Dept Phys, Phys Soc Japan, Scholast Inc, Stanford Univ, Thomas Jefferson Natl Accelerator Facil, UNESCO, Univ Dist Columbia, Univ Penn, Dept Phys & Astronomy, Dept Sci & Technol, Council Sci & Ind Res (Def Peace Safety & Secur; Mat Sci & Mfg; R&D; R&D Outcomes & Human Capital Dev), Juta Publishers, Natl Res Fdn, Nelson Mandela Metropolitan Univ, Dept Phys, S African Agcy Sci & Technol Awareness, S African Inst Phys, Square Kilometre Array Africa, Univ Pretoria, Dept Phys C1 [Seestrom, Susan J.] Los Alamos Natl Lab, UCNA Collaborat, Los Alamos, NM USA. NR 0 TC 0 Z9 0 U1 1 U2 2 PU AMER INST PHYSICS PI MELVILLE PA 2 HUNTINGTON QUADRANGLE, STE 1NO1, MELVILLE, NY 11747-4501 USA SN 0094-243X BN 978-0-7354-1138-8 J9 AIP CONF PROC PY 2013 VL 1517 BP 201 EP 201 PG 1 WC Physics, Applied SC Physics GA BEK11 UT WOS:000317018600121 ER PT S AU Petreczky, P AF Petreczky, Peter BE Goncalves, VP DaSilva, MLL Amaral, JTD Machado, MVT TI QCD at non-zero temperature : status and prospects SO XII HADRON PHYSICS SE AIP Conference Proceedings LA English DT Proceedings Paper CT 12th Hadron Physics Conference CY APR 22-27, 2012 CL Bento Goncalves, BRAZIL SP CNPq, CAPES, CLAF, FAPESP, FAPERJ, FAPERGS, FAPEMIG, UFRGS DE Lattice QCD; Quark Gluon Plasma; Hadron Resonance Gas ID QUARK-GLUON PLASMA; SU(2) GAUGE-THEORY; YANG-MILLS THEORY; MESON SPECTRAL FUNCTIONS; DECONFINEMENT PHASE-TRANSITION; MAXIMUM-ENTROPY ANALYSIS; SPATIAL STRING TENSION; CHIRAL CRITICAL-POINT; ADJOINT HIGGS-MODEL; FINITE-TEMPERATURE AB I will discuss recent progress in lattice QCD calculations related to the QCD phase diagram, equation of state and meson spectral functions. C1 Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. RP Petreczky, P (reprint author), Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. NR 212 TC 6 Z9 6 U1 0 U2 0 PU AMER INST PHYSICS PI MELVILLE PA 2 HUNTINGTON QUADRANGLE, STE 1NO1, MELVILLE, NY 11747-4501 USA SN 0094-243X BN 978-0-7354-1143-2 J9 AIP CONF PROC PY 2013 VL 1520 BP 103 EP 147 DI 10.1063/1.4795947 PG 45 WC Physics, Nuclear SC Physics GA BES88 UT WOS:000317972900004 ER PT S AU Fazio, S AF Fazio, Salvatore BE Goncalves, VP DaSilva, MLL Amaral, JTD Machado, MVT TI DVCS and GPDs at eRHIC: towards a high resolution partonic imaging SO XII HADRON PHYSICS SE AIP Conference Proceedings LA English DT Proceedings Paper CT 12th Hadron Physics Conference CY APR 22-27, 2012 CL Bento Goncalves, BRAZIL SP CNPq, CAPES, CLAF, FAPESP, FAPERJ, FAPERGS, FAPEMIG, UFRGS DE DVCS; GPDs; eRHIC; EIC AB The feasibility for a measurement of the exclusive production of a real photon, a process although known as Deeply Virtual Compton Scattering (DVCS) at an eRHIC has been explored. An electron-proton/ion collider facility (eRHIC) is under consideration at Brookhaven National Laboratory (BNL). Such a new facility will require the design and construction of a new optimized detector profiting from the experience gained from electron-proton colliders like at the experiments H1 and ZEUS at DESY-HERA. In particular, eRHIC is a machine designed to collide an electron beam with energies ranging from 5 GeV up to 20 GeV with the RHIC hadron beams (protons (100-250 GeV) and nuclei (<= 100 GeV)), thus varying center-of-mass energies. DVCS is universally believed to be a golden measurement toward the determination of the Generalized Parton Distribution (GPDs) functions. The high luminosity of the machine, expected in the order of 10(34) cm(2)s(-1) at the highest center-of-mass energy, together with the large rapidity acceptance of a newly designed dedicated detector, will open the opportunity for measuring DVCS with an unprecedented precision, providing an important tool toward a 2+1 dimensional picture of the internal structure of the proton. The huge impact such measurements would have on the determination of GPDs will be discussed. C1 Brookhaven Natl Lab, Upton, NY 11973 USA. RP Fazio, S (reprint author), Brookhaven Natl Lab, POB 5000, Upton, NY 11973 USA. RI Fazio, Salvatore /G-5156-2010 NR 4 TC 0 Z9 0 U1 0 U2 2 PU AMER INST PHYSICS PI MELVILLE PA 2 HUNTINGTON QUADRANGLE, STE 1NO1, MELVILLE, NY 11747-4501 USA SN 0094-243X BN 978-0-7354-1143-2 J9 AIP CONF PROC PY 2013 VL 1520 BP 154 EP 159 DI 10.1063/1.4795949 PG 6 WC Physics, Nuclear SC Physics GA BES88 UT WOS:000317972900006 ER PT S AU Koch, V Bzdak, A Skokov, V AF Koch, Volker Bzdak, Adam Skokov, Vladimir BE Goncalves, VP DaSilva, MLL Amaral, JTD Machado, MVT TI Fluctuations and the QCD Phase Diagram SO XII HADRON PHYSICS SE AIP Conference Proceedings LA English DT Proceedings Paper CT 12th Hadron Physics Conference CY APR 22-27, 2012 CL Bento Goncalves, BRAZIL SP CNPq, CAPES, CLAF, FAPESP, FAPERJ, FAPERGS, FAPEMIG, UFRGS DE QCD; Fluctuations; Phase Diagram ID TRANSITION AB We briefly review how fluctuation measurements may help to reveal the properties of the QCD phase diagram. We further discuss various background effects, such as charge conservation, which contribute to fluctuation observables and which need to be well understood before definitive conclusions about a possible phase structure can be drawn. C1 [Koch, Volker] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Bzdak, Adam] RIKEN BNL Res Ctr, Brookhaven Natl Lab, Upton, NY 11973 USA. [Skokov, Vladimir] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. RP Koch, V (reprint author), Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. OI Skokov, Vladimir/0000-0001-7619-1796 FU U. S. Department of Energy [DE-AC02-98CH10886]; Office of Nuclear Physics in the US Department of Energy's Ofce of Science [DE-AC02-05CH11231]; Polish Ministry of Science and Higher Education [N202 125437] FX A. B. and V. S. were supported by Contract No. DE-AC02-98CH10886 with the U. S. Department of Energy. V. K. was supported by the Office of Nuclear Physics in the US Department of Energys Ofce of Science under Contract No. DE-AC02-05CH11231. A. B. also acknowledges the grant N N202 125437 of the Polish Ministry of Science and Higher Education (2009-2012). NR 17 TC 0 Z9 0 U1 0 U2 0 PU AMER INST PHYSICS PI MELVILLE PA 2 HUNTINGTON QUADRANGLE, STE 1NO1, MELVILLE, NY 11747-4501 USA SN 0094-243X BN 978-0-7354-1143-2 J9 AIP CONF PROC PY 2013 VL 1520 BP 232 EP 237 DI 10.1063/1.4795962 PG 6 WC Physics, Nuclear SC Physics GA BES88 UT WOS:000317972900019 ER PT S AU de Urreta, EJG Scoccola, NN Jayalath, CP Goity, JL AF Gonzalez de Urreta, E. J. Scoccola, N. N. Jayalath, C. P. Goity, J. L. BE Goncalves, VP DaSilva, MLL Amaral, JTD Machado, MVT TI Partial Decay Widths of Negative Parity Baryons in the 1/N-c Expansion SO XII HADRON PHYSICS SE AIP Conference Proceedings LA English DT Proceedings Paper CT 12th Hadron Physics Conference CY APR 22-27, 2012 CL Bento Goncalves, BRAZIL SP CNPq, CAPES, CLAF, FAPESP, FAPERJ, FAPERGS, FAPEMIG, UFRGS DE Large N-c QCD; excited baryons ID LARGE N-C; QCD; MASSES AB The partial decay widths of lowest lying negative parity baryons belonging to the 70-plet of SU(6) are analyzed in the framework of the 1/N-c expansion. The channels considered are those with single pseudoscalar meson emission. The analysis is carried out to sub-leading order in 1/N-c and to first order in SU(3) symmetry breaking. Conclusions about the magnitude of SU(3) breaking effects along with predictions for some unknown or poorly determined partial decay widths of known resonances are given. C1 [Gonzalez de Urreta, E. J.; Scoccola, N. N.] CNEA, Ctr Atom Constituyentes, Dept Phys, Buenos Aires, DF, Argentina. [Scoccola, N. N.] Univ Favaloro, Buenos Aires, DF, Argentina. [Jayalath, C. P.; Goity, J. L.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. [Jayalath, C. P.] Univ Peradeniya, Dept Phys, Peradeniya 20400, Sri Lanka. RP de Urreta, EJG (reprint author), CNEA, Ctr Atom Constituyentes, Dept Phys, Buenos Aires, DF, Argentina. FU DOE [DE-AC05-06OR23177]; JSA operates the Thomas Jefferson National Accelerator Facility; National Science Foundation (USA) [PHY-0555559, PHY-0855789]; CONICET [PIP 02368]; ANPCyT [PICT 07-03-00818] FX EGU and NNS wants to thank the organizers for their warm hospitality during the workshop. This work was supported by DOE Contract No. DE-AC05-06OR23177 under which JSA operates the Thomas Jefferson National Accelerator Facility, by the National Science Foundation (USA) through grant PHY-0555559 and PHY-0855789 (JLG and CJ), by CONICET (Argentina) grant # PIP 02368 and by ANPCyT (Argentina) grants PICT 07-03-00818 (EGU and NNS). NR 23 TC 0 Z9 0 U1 0 U2 0 PU AMER INST PHYSICS PI MELVILLE PA 2 HUNTINGTON QUADRANGLE, STE 1NO1, MELVILLE, NY 11747-4501 USA SN 0094-243X BN 978-0-7354-1143-2 J9 AIP CONF PROC PY 2013 VL 1520 BP 249 EP 254 DI 10.1063/1.4795965 PG 6 WC Physics, Nuclear SC Physics GA BES88 UT WOS:000317972900022 ER PT J AU Bar-Shalom, S Geller, M Nandi, S Soni, A AF Bar-Shalom, Shaouly Geller, Michael Nandi, Soumitra Soni, Amarjit TI Two Higgs Doublets, a 4th Generation and a 125 GeV Higgs: A Review SO ADVANCES IN HIGH ENERGY PHYSICS LA English DT Review ID ELECTROWEAK SYMMETRY-BREAKING; LEADING QCD CORRECTIONS; ULTRA HEAVY FERMIONS; STANDARD-MODEL; TOP-QUARK; WEAK-INTERACTIONS; BARYON ASYMMETRY; FLAVOR VIOLATION; COMPOSITE HIGGS; PP COLLISIONS AB We review the possible role that multi-Higgs models may play in our understanding of the dynamics of a heavy 4th sequential generation of fermions. We describe the underlying ingredients of such models, focusing on two Higgs doublets, and discuss how they may effectively accommodate the low-energy phenomenology of such new heavy fermionic degrees of freedom. We also discuss the constraints on these models from precision electroweak data as well as from flavor physics and the implications for collider searches of the Higgs particles and of the 4th generation fermions, bearing in mind the recent observation of a light Higgs with a mass of similar to 125GeV. C1 [Bar-Shalom, Shaouly; Geller, Michael] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Nandi, Soumitra] Univ Siegen, Nat Wissensch Tech Fak, D-57068 Siegen, Germany. [Nandi, Soumitra] Indian Inst Technol, Gauhati 781039, Assam, India. [Soni, Amarjit] Brookhaven Natl Lab, Theory Grp, Upton, NY 11973 USA. RP Nandi, S (reprint author), Univ Siegen, Nat Wissensch Tech Fak, D-57068 Siegen, Germany. EM soumitra.nandi@gmail.com OI nandi, soumitra/0000-0001-6567-0302 FU Technion; U.S. DOE [DE-AC02-98CH10886(BNL)] FX SBS and MG acknowledge research support from the Technion. The work of AS was supported in part by the U.S. DOE Contract no. DE-AC02-98CH10886(BNL). NR 155 TC 3 Z9 3 U1 0 U2 2 PU HINDAWI PUBLISHING CORPORATION PI NEW YORK PA 410 PARK AVENUE, 15TH FLOOR, #287 PMB, NEW YORK, NY 10022 USA SN 1687-7357 EI 1687-7365 J9 ADV HIGH ENERGY PHYS JI Adv. High. Energy Phys. PY 2013 AR 672972 DI 10.1155/2013/672972 PG 28 WC Physics, Particles & Fields SC Physics GA 132UD UT WOS:000318093300001 ER PT J AU Martin del Campo, JS Rollin, J Myung, S Chun, Y Chandrayan, S Patino, R Adams, MWW Zhang, YHP AF Martin del Campo, Julia S. Rollin, Joseph Myung, Suwan Chun, You Chandrayan, Sanjeev Patino, Rodrigo Adams, Michael W. W. Zhang, Y. -H. Percival TI High-Yield Production of Dihydrogen from Xylose by Using a Synthetic Enzyme Cascade in a Cell-Free System SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE biocatalysis; hydrogen; hydrogenases; polyphosphates; xylose ID FERMENTATIVE HYDROGEN-PRODUCTION; ESCHERICHIA-COLI; BIOMASS; WATER; GLUCOSE; BIOHYDROGEN; STARCH C1 [Martin del Campo, Julia S.; Rollin, Joseph; Myung, Suwan; Chun, You; Zhang, Y. -H. Percival] Virginia Tech, Dept Biol Syst Engn, Blacksburg, VA 24061 USA. [Martin del Campo, Julia S.; Patino, Rodrigo] Ctr Invest & Estudios Avanzados, Dept Fis Aplicada, Merida 97310, Yucatan, Mexico. [Chandrayan, Sanjeev; Adams, Michael W. W.] Univ Georgia, Dept Biochem & Mol Biol, Athens, GA 30602 USA. [Myung, Suwan; Zhang, Y. -H. Percival] Virginia Tech, ICTAS, Blacksburg, VA 24061 USA. [Adams, Michael W. W.; Zhang, Y. -H. Percival] DOE BioEnergy Sci Ctr BESC, Oak Ridge, TN 37831 USA. RP Zhang, YHP (reprint author), Virginia Tech, Dept Biol Syst Engn, Blacksburg, VA 24061 USA. EM ypzhang@vt.edu RI You, Chun/D-7656-2013; CHANDRAYAN, SANJEEV /M-1662-2016 OI CHANDRAYAN, SANJEEV /0000-0003-2219-4654 FU Biological Systems Engineering Department of Virginia Tech; Shell GameChanger Program; CALS Biodesign and Bioprocessing Research Center; DOE BioEnergy Science Center; Division of Chemical Sciences, Geosciences and Biosciences, Office of Basic Energy Sciences of the DOE [DE-FG05-95ER20175]; Mexican Council of Science and Technology (Conacyt) FX This work was supported by the Biological Systems Engineering Department of Virginia Tech, and partially supported by Shell GameChanger Program, the CALS Biodesign and Bioprocessing Research Center, and the DOE BioEnergy Science Center (to P.Z.) and the Division of Chemical Sciences, Geosciences and Biosciences, Office of Basic Energy Sciences of the DOE (DE-FG05-95ER20175 to M.A.). JSMC thanked the Mexican Council of Science and Technology (Conacyt) for her PhD grant. NR 31 TC 14 Z9 14 U1 3 U2 76 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PY 2013 VL 52 IS 17 BP 4587 EP 4590 DI 10.1002/anie.201300766 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA 132BU UT WOS:000318043600013 PM 23512726 ER PT J AU Boukhalfa, S He, L Melnichenko, YB Yushin, G AF Boukhalfa, S. He, L. Melnichenko, Y. B. Yushin, Gleb TI Small-Angle Neutron Scattering for InSitu Probing of Ion Adsorption Inside Micropores SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE adsorption; carbon; energy storage; nanoporous materials; small-angle neutron scattering ID DOUBLE-LAYER CAPACITORS; CARBON NANOTUBE; ENERGY-STORAGE; ELECTRODES; SUPERCAPACITORS; ELECTROLYTES; DEPOSITION; OXIDE C1 [Boukhalfa, S.; Yushin, Gleb] Georgia Inst Technol, Sch Mat Sci & Engn, Atlanta, GA 30332 USA. [He, L.; Melnichenko, Y. B.] Oak Ridge Natl Lab, Neutron Sci Directorate, Biol & Soft Matter Div, Oak Ridge, TN USA. [Melnichenko, Y. B.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37966 USA. RP Yushin, G (reprint author), Georgia Inst Technol, Sch Mat Sci & Engn, Atlanta, GA 30332 USA. EM yushin@gatech.edu RI Yushin, Gleb/B-4529-2013; OI Yushin, Gleb/0000-0002-3274-9265; He, Lilin/0000-0002-9560-8101 FU Georgia Institute of Technology; US Army Research Office [W911NF-12-1-0259]; Laboratory Directed Research and Development Program; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; ORNL Postdoctoral Research Associates Program FX This work was partially supported by the Georgia Institute of Technology and the US Army Research Office (contract number W911NF-12-1-0259). The research at ORNL's High Flux Isotope Reactor was sponsored by the Laboratory Directed Research and Development Program and the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. This research was also supported in part by the ORNL Postdoctoral Research Associates Program, administered jointly by the ORNL and the Oak Ridge Institute for Science and Education. We thank Micromeritics Inc. (US) and J. Jagiello for assistance with gas and vapor sorption analyses. NR 29 TC 16 Z9 16 U1 2 U2 52 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PY 2013 VL 52 IS 17 BP 4618 EP 4622 DI 10.1002/anie.201209141 PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA 132BU UT WOS:000318043600020 PM 23364852 ER PT J AU Shindell, DT Lamarque, JF Schulz, M Flanner, M Jiao, C Chin, M Young, PJ Lee, YH Rotstayn, L Mahowald, N Milly, G Faluvegi, G Balkanski, Y Collins, WJ Conley, AJ Dalsoren, S Easter, R Ghan, S Horowitz, L Liu, X Myhre, G Nagashima, T Naik, V Rumbold, ST Skeie, R Sudo, K Szopa, S Takemura, T Voulgarakis, A Yoon, JH Lo, F AF Shindell, D. T. Lamarque, J. -F. Schulz, M. Flanner, M. Jiao, C. Chin, M. Young, P. J. Lee, Y. H. Rotstayn, L. Mahowald, N. Milly, G. Faluvegi, G. Balkanski, Y. Collins, W. J. Conley, A. J. Dalsoren, S. Easter, R. Ghan, S. Horowitz, L. Liu, X. Myhre, G. Nagashima, T. Naik, V. Rumbold, S. T. Skeie, R. Sudo, K. Szopa, S. Takemura, T. Voulgarakis, A. Yoon, J. -H. Lo, F. TI Radiative forcing in the ACCMIP historical and future climate simulations SO ATMOSPHERIC CHEMISTRY AND PHYSICS LA English DT Article ID INTERCOMPARISON PROJECT ACCMIP; COMMUNITY ATMOSPHERE MODEL; BLACK CARBON; SYSTEM MODEL; AEROSOL; PREINDUSTRIAL; CHEMISTRY; SENSITIVITY; DISTRIBUTIONS; EMISSIONS AB The Atmospheric Chemistry and Climate Model Intercomparison Project (ACCMIP) examined the short-lived drivers of climate change in current climate models. Here we evaluate the 10 ACCMIP models that included aerosols, 8 of which also participated in the Coupled Model Intercomparison Project phase 5 (CMIP5). The models reproduce present-day total aerosol optical depth (AOD) relatively well, though many are biased low. Contributions from individual aerosol components are quite different, however, and most models underestimate east Asian AOD. The models capture most 1980-2000 AOD trends well, but underpredict increases over the Yellow/Eastern Sea. They strongly underestimate absorbing AOD in many regions. We examine both the direct radiative forcing (RF) and the forcing including rapid adjustments (effective radiative forcing; ERF, including direct and indirect effects). The models' all-sky 1850 to 2000 global mean annual average total aerosol RF is (mean; range) -0.26 Wm(-2); -0.06 to -0.49 Wm(-2). Screening based on model skill in capturing observed AOD yields a best estimate of -0.42 Wm(-2); -0.33 to -0.50 Wm(-2), including adjustment for missing aerosol components in some models. Many ACCMIP and CMIP5 models appear to produce substantially smaller aerosol RF than this best estimate. Climate feedbacks contribute substantially (35 to -58%) to modeled historical aerosol RF. The 1850 to 2000 aerosol ERF is -1.17 Wm(-2); -0.71 to -1.44 Wm(-2). Thus adjustments, including clouds, typically cause greater forcing than direct RF. Despite this, the multi-model spread relative to the mean is typically the same for ERF as it is for RF, or even smaller, over areas with substantial forcing. The largest 1850 to 2000 negative aerosol RF and ERF values are over and near Europe, south and east Asia and North America. ERF, however, is positive over the Sahara, the Karakoram, high Southern latitudes and especially the Arctic. Global aerosol RF peaks in most models around 1980, declining thereafter with only weak sensitivity to the Representative Concentration Pathway (RCP). One model, however, projects approximately stable RF levels, while two show increasingly negative RF due to nitrate (not included in most models). Aerosol ERF, in contrast, becomes more negative during 1980 to 2000. During this period, increased Asian emissions appear to have a larger impact on aerosol ERF than European and North American decreases due to their being upwind of the large, relatively pristine Pacific Ocean. There is no clear relationship between historical aerosol ERF and climate sensitivity in the CMIP5 subset of ACCMIP models. In the ACCMIP/CMIP5 models, historical aerosol ERF of about -0.8 to -1.5 Wm(-2) is most consistent with observed historical warming. Aerosol ERF masks a large portion of greenhouse forcing during the late 20th and early 21st century at the global scale. Regionally, aerosol ERF is so large that net forcing is negative over most industrialized and biomass burning regions through 1980, but remains strongly negative only over east and southeast Asia by 2000. Net forcing is strongly positive by 1980 over most deserts, the Arctic, Australia, and most tropical oceans. Both the magnitude of and area covered by positive forcing expand steadily thereafter. C1 [Shindell, D. T.; Lee, Y. H.; Milly, G.; Faluvegi, G.; Voulgarakis, A.] NASA, Goddard Inst Space Studies, New York, NY 10025 USA. [Shindell, D. T.; Lee, Y. H.; Milly, G.; Faluvegi, G.; Voulgarakis, A.] Columbia Earth Inst, New York, NY USA. [Lamarque, J. -F.; Conley, A. J.] Natl Ctr Atmospher Res, Boulder, CO 80307 USA. [Schulz, M.] Inst Meteorol, Oslo, Norway. [Flanner, M.; Jiao, C.] Univ Michigan, Dept Atmospher Ocean & Space Sci, Ann Arbor, MI 48109 USA. [Chin, M.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Young, P. J.] Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA. [Young, P. J.] NOAA, Earth Syst Res Lab, Boulder, CO USA. [Rotstayn, L.] CSIRO Marine & Atmospher Res, Ctr Australian Weather & Climate Res, Aspendale, Vic, Australia. [Mahowald, N.; Lo, F.] Cornell Univ, Dept Earth & Atmospher Sci, Ithaca, NY USA. [Balkanski, Y.; Szopa, S.] IPSL, LSCE, Gif Sur Yvette, France. [Collins, W. J.; Rumbold, S. T.] Hadley Ctr, Met Off, Exeter, Devon, England. [Dalsoren, S.; Myhre, G.; Skeie, R.] CICERO, Oslo, Norway. [Easter, R.; Ghan, S.; Liu, X.; Yoon, J. -H.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Horowitz, L.] NOAA, Geophys Fluid Dynam Lab, Princeton, NJ USA. [Nagashima, T.] Natl Inst Environm Studies, Tsukuba, Ibaraki, Japan. [Naik, V.] NOAA, UCAR, Geophys Fluid Dynam Lab, Princeton, NJ USA. [Sudo, K.] Nagoya Univ, Grad Sch Environm Studies, Dept Earth & Environm Sci, Nagoya, Aichi 4648601, Japan. [Takemura, T.] Kyushu Univ, Appl Mech Res Inst, Fukuoka 8168580, Japan. [Voulgarakis, A.] Univ London Imperial Coll Sci Technol & Med, Dept Phys, London, England. RP Shindell, DT (reprint author), NASA, Goddard Inst Space Studies, New York, NY 10025 USA. EM drew.t.shindell@nasa.gov RI Balkanski, Yves/A-6616-2011; Lamarque, Jean-Francois/L-2313-2014; Kyushu, RIAM/F-4018-2015; Jiao, Chaoyi/F-9065-2015; Myhre, Gunnar/A-3598-2008; Skeie, Ragnhild/K-1173-2015; Schulz, Michael/A-6930-2011; U-ID, Kyushu/C-5291-2016; Ghan, Steven/H-4301-2011; Lee, Yunha/Q-7222-2016; Manager, CSD Publications/B-2789-2015; Collins, William/A-5895-2010; Takemura, Toshihiko/C-2822-2009; Young, Paul/E-8739-2010; Flanner, Mark/C-6139-2011; Mahowald, Natalie/D-8388-2013; Horowitz, Larry/D-8048-2014; Naik, Vaishali/A-4938-2013; YOON, JIN-HO/A-1672-2009; Liu, Xiaohong/E-9304-2011; Rotstayn, Leon/A-1756-2012; Szopa, Sophie/F-8984-2010; Chin, Mian/J-8354-2012; Shindell, Drew/D-4636-2012 OI Balkanski, Yves/0000-0001-8241-2858; Lamarque, Jean-Francois/0000-0002-4225-5074; Myhre, Gunnar/0000-0002-4309-476X; Skeie, Ragnhild/0000-0003-1246-4446; Schulz, Michael/0000-0003-4493-4158; Ghan, Steven/0000-0001-8355-8699; Lee, Yunha/0000-0001-7478-2672; Collins, William/0000-0002-7419-0850; Takemura, Toshihiko/0000-0002-2859-6067; Young, Paul/0000-0002-5608-8887; Flanner, Mark/0000-0003-4012-174X; Mahowald, Natalie/0000-0002-2873-997X; Horowitz, Larry/0000-0002-5886-3314; Naik, Vaishali/0000-0002-2254-1700; YOON, JIN-HO/0000-0002-4939-8078; Liu, Xiaohong/0000-0002-3994-5955; Rotstayn, Leon/0000-0002-2385-4223; Szopa, Sophie/0000-0002-8641-1737; FU NASA MAP program; ACMAP program; NASA High-End Computing (HEC) Program through the NASA Center for Climate Simulation (NCCS); National Science Foundation; Office of Science (BER) of the US Department of Energy; US Department of Energy Office of Science Decadal and Regional Climate Prediction; DOE by Battelle Memorial Institute [DE-AC06-76RLO 1830]; Joint DECC and Defra Integrated Climate Programme [GA01101]; Environment Research and Technology Development Fund of the Ministry of the Environment, Japan [S-7]; Norwegian Research Council; Atmospheric Chemistry and Climate (ACC); project of International Global Atmospheric Chemistry (IGAC); Stratospheric Processes And their Role in Climate (SPARC) under the International Geosphere-Biosphere Project (IGBP); World Climate Research Program (WCRP) FX Thanks to Stephen Jeffrey for assistance with data analysis. We acknowledge the World Climate Research Programme's Working Group on Coupled Modelling, which is responsible for CMIP, and the US Department of Energy's Program for Climate Model Diagnosis and Intercomparison, and we thank the climate modeling groups (listed in Tables 1, G1 and G2 of this paper) for producing and making available their model output as well as the satellite data teams. The authors are grateful to the British Atmospheric Data Centre (BADC) for collecting and archiving the ACCMIP data. DS acknowledges support from the NASA MAP and ACMAP programs and the NASA High-End Computing (HEC) Program through the NASA Center for Climate Simulation (NCCS). The CESM project is supported by the National Science Foundation and the Office of Science (BER) of the US Department of Energy. The National Center for Atmospheric Research is operated by the University Corporation for Atmospheric Research under sponsorship of the National Science Foundation. S. Ghan was supported by the US Department of Energy Office of Science Decadal and Regional Climate Prediction using Earth System Models (EaSM) program. The Pacific Northwest National Laboratory (PNNL) is operated for the DOE by Battelle Memorial Institute under contract DE-AC06-76RLO 1830. W. J. Collins and S. T. Rumbold were supported by the Joint DECC and Defra Integrated Climate Programme (GA01101). VN and LWH acknowledge efforts of GFDL's Global Atmospheric Model Development Team in the development of the GFDL-AM3 and Modeling Services Group for assistance with data processing. The MIROC-CHEM calculations were performed on the NIES supercomputer system (NEC SX-8R), and supported by the Environment Research and Technology Development Fund (S-7) of the Ministry of the Environment, Japan. The LMDz-OR-INCA simulations were done using computing resources provided by the CCRT/GENCI computer center of the CEA. The CICERO-OsloCTM2 simulations were done within the projects SLAC (Short Lived Atmospheric Components) and EarthClim funded by the Norwegian Research Council. ACCMIP is organized under the auspices of Atmospheric Chemistry and Climate (AC&C), a project of International Global Atmospheric Chemistry (IGAC) and Stratospheric Processes And their Role in Climate (SPARC) under the International Geosphere-Biosphere Project (IGBP) and World Climate Research Program (WCRP). NR 78 TC 141 Z9 144 U1 8 U2 95 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1680-7316 EI 1680-7324 J9 ATMOS CHEM PHYS JI Atmos. Chem. Phys. PY 2013 VL 13 IS 6 BP 2939 EP 2974 DI 10.5194/acp-13-2939-2013 PG 36 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 117NU UT WOS:000316961000002 ER PT J AU Stevenson, DS Young, PJ Naik, V Lamarque, JF Shindell, DT Voulgarakis, A Skeie, RB Dalsoren, SB Myhre, G Berntsen, TK Folberth, GA Rumbold, ST Collins, WJ MacKenzie, IA Doherty, RM Zeng, G van Noije, TPC Strunk, A Bergmann, D Cameron-Smith, P Plummer, DA Strode, SA Horowitz, L Lee, YH Szopa, S Sudo, K Nagashima, T Josse, B Cionni, I Righi, M Eyring, V Conley, A Bowman, KW Wild, O Archibald, A AF Stevenson, D. S. Young, P. J. Naik, V. Lamarque, J. -F. Shindell, D. T. Voulgarakis, A. Skeie, R. B. Dalsoren, S. B. Myhre, G. Berntsen, T. K. Folberth, G. A. Rumbold, S. T. Collins, W. J. MacKenzie, I. A. Doherty, R. M. Zeng, G. van Noije, T. P. C. Strunk, A. Bergmann, D. Cameron-Smith, P. Plummer, D. A. Strode, S. A. Horowitz, L. Lee, Y. H. Szopa, S. Sudo, K. Nagashima, T. Josse, B. Cionni, I. Righi, M. Eyring, V. Conley, A. Bowman, K. W. Wild, O. Archibald, A. TI Tropospheric ozone changes, radiative forcing and attribution to emissions in the Atmospheric Chemistry and Climate Model Intercomparison Project (ACCMIP) SO ATMOSPHERIC CHEMISTRY AND PHYSICS LA English DT Article ID LONG-TERM CHANGES; SURFACE OZONE; PREINDUSTRIAL TIMES; STRATOSPHERIC OZONE; GLOBAL ATMOSPHERE; GREENHOUSE GASES; NITROGEN-OXIDES; 3-D MODELS; METHANE; AIR AB Ozone (O-3) from 17 atmospheric chemistry models taking part in the Atmospheric Chemistry and Climate Model Intercomparison Project (ACCMIP) has been used to calculate tropospheric ozone radiative forcings (RFs). All models applied a common set of anthropogenic emissions, which are better constrained for the present-day than the past. Future anthropogenic emissions follow the four Representative Concentration Pathway (RCP) scenarios, which define a relatively narrow range of possible air pollution emissions. We calculate a value for the pre-industrial (1750) to present-day (2010) tropospheric ozone RF of 410 mW m(-2). The model range of pre-industrial to present-day changes in O-3 produces a spread (+/- 1 standard deviation) in RFs of +/- 17 %. Three different radiation schemes were used we find differences in RFs between schemes (for the same ozone fields) of +/- 10 %. Applying two different tropopause definitions gives differences in RFs of +/- 3 %. Given additional (unquantified) uncertainties associated with emissions, climate-chemistry interactions and land-use change, we estimate an overall uncertainty of +/- 30% for the tropospheric ozone RF. Experiments carried out by a subset of six models attribute tropospheric ozone RF to increased emissions of methane (44 +/- 12 %), nitrogen oxides (31 +/- 9 %), carbon monoxide (15 +/- 3 %) and non-methane volatile organic compounds (9 +/- 2 %); earlier studies attributed more of the tropospheric ozone RF to methane and less to nitrogen oxides. Normalising RFs to changes in tropospheric column ozone, we find a global mean normalised RF of 42 mW m(-2) DU-1, a value similar to previous work. Using normalised RFs and future tropospheric column ozone projections we calculate future tropospheric ozone RFs (mW m(-2); relative to 1750) for the four future scenarios (RCP2.6, RCP4.5, RCP6.0 and RCP8.5) of 350, 420, 370 and 460 (in 2030), and 200, 300, 280 and 600 (in 2100). Models show some coherent responses of ozone to climate change: decreases in the tropical lower troposphere, associated with increases in water vapour; and increases in the sub-tropical to mid-latitude upper troposphere, associated with increases in lightning and stratosphere-to-troposphere transport. Climate change has relatively small impacts on global mean tropospheric ozone RF. C1 [Stevenson, D. S.; MacKenzie, I. A.; Doherty, R. M.] Univ Edinburgh, Sch Geosci, Edinburgh, Midlothian, Scotland. [Young, P. J.] NOAA, Div Chem Sci, Earth Syst Res Lab, Boulder, CO USA. [Young, P. J.] Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA. [Naik, V.] NOAA, UCAR, Geophys Fluid Dynam Lab, Princeton, NJ USA. [Lamarque, J. -F.; Conley, A.] Natl Ctr Atmospher Res, Boulder, CO 80307 USA. [Shindell, D. T.; Lee, Y. H.] NASA, Goddard Inst Space Studies, New York, NY 10025 USA. [Shindell, D. T.; Lee, Y. H.] Columbia Earth Inst, New York, NY USA. [Voulgarakis, A.] Univ London Imperial Coll Sci Technol & Med, Dept Phys, London, England. [Skeie, R. B.; Dalsoren, S. B.; Myhre, G.; Berntsen, T. K.] CICERO, Oslo, Norway. [Folberth, G. A.; Rumbold, S. T.; Collins, W. J.] Met Off Hadley Ctr, Exeter, Devon, England. [Zeng, G.] Natl Inst Water & Atmospher Res, Lauder, New Zealand. [van Noije, T. P. C.; Strunk, A.] Royal Netherlands Meteorol Inst, NL-3730 AE De Bilt, Netherlands. [Bergmann, D.; Cameron-Smith, P.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Plummer, D. A.] Environm Canada, Canadian Ctr Climate Modeling & Anal, Victoria, BC, Canada. [Strode, S. A.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Strode, S. A.] Univ Space Res Assoc, Columbia, MD USA. [Horowitz, L.] NOAA, Geophys Fluid Dynam Lab, Princeton, NJ USA. [Szopa, S.] Lab Sci Climat & Environm, Gif Sur Yvette, France. [Sudo, K.] Nagoya Univ, Grad Sch Environm Studies, Dept Earth & Environm Sci, Nagoya, Aichi 4648601, Japan. [Nagashima, T.] Natl Inst Environm Studies, Tsukuba, Ibaraki, Japan. [Josse, B.] CNRS Ctr Natl Rech Meteorol, CNRM, GAME, Toulouse, France. [Cionni, I.] Agenzia Nazl Nuove Tecnol Energia & Sviluppo Econ, Bologna, Italy. [Righi, M.; Eyring, V.] Deutsch Zentrum Luft & Raumfahrt DLR, Inst Phys Atmosphare, Oberpfaffenhofen, Germany. [Bowman, K. W.] NASA, Jet Prop Lab, Pasadena, CA USA. [Wild, O.] Univ Lancaster, Lancaster Environm Ctr, Lancaster, England. [Archibald, A.] Univ Cambridge, Ctr Atmospher Sci, Cambridge CB2 1TN, England. RP Stevenson, DS (reprint author), Univ Edinburgh, Sch Geosci, Edinburgh, Midlothian, Scotland. EM david.s.stevenson@ed.ac.uk RI Skeie, Ragnhild/K-1173-2015; Strode, Sarah/H-2248-2012; Eyring, Veronika/O-9999-2016; Lee, Yunha/Q-7222-2016; Manager, CSD Publications/B-2789-2015; Cameron-Smith, Philip/E-2468-2011; Szopa, Sophie/F-8984-2010; Shindell, Drew/D-4636-2012; Horowitz, Larry/D-8048-2014; Bergmann, Daniel/F-9801-2011; Naik, Vaishali/A-4938-2013; Lamarque, Jean-Francois/L-2313-2014; Myhre, Gunnar/A-3598-2008; Stevenson, David/C-8089-2012; Collins, William/A-5895-2010; Young, Paul/E-8739-2010; Wild, Oliver/A-4909-2009; Righi, Mattia/I-5120-2013 OI Righi, Mattia/0000-0003-3827-5950; Skeie, Ragnhild/0000-0003-1246-4446; Strode, Sarah/0000-0002-8103-1663; Eyring, Veronika/0000-0002-6887-4885; Lee, Yunha/0000-0001-7478-2672; Archibald, Alexander/0000-0001-9302-4180; Folberth, Gerd/0000-0002-1075-440X; Cameron-Smith, Philip/0000-0002-8802-8627; Szopa, Sophie/0000-0002-8641-1737; Horowitz, Larry/0000-0002-5886-3314; Bergmann, Daniel/0000-0003-4357-6301; Naik, Vaishali/0000-0002-2254-1700; Lamarque, Jean-Francois/0000-0002-4225-5074; Myhre, Gunnar/0000-0002-4309-476X; Stevenson, David/0000-0002-4745-5673; Collins, William/0000-0002-7419-0850; Young, Paul/0000-0002-5608-8887; Wild, Oliver/0000-0002-6227-7035; FU Atmospheric Chemistry and Climate (ACC); Joint DECC and Defra Integrated Climate Programme [GA01101]; Defra SSNIP air quality contract [AQ 0902]; New Zealand Ministry of Science and Innovation; National Science Foundation; Office of Science (BER) of the US Department of Energy; US Dept. of Energy (BER); LLNL [DE-AC52-07NA27344]; NERSC [DE-AC02-05CH11231]; NASA Modeling, Analysis and Prediction program; Environment Research and Technology Development Fund of the Ministry of the Environment, Japan [S-7]; Office of Science and Technology through EPSRC's High End Computing Programme; Norwegian Research Council; Meteo-France; CNRS; NASA MAP program; NASA ACMAP program; SciDAC program of the Dept. of Energy; UK Met Office; NOAA; CICERO; NIWA; Edinburgh University FX ACCMIP is organized under the auspices of Atmospheric Chemistry and Climate (AC&C), a project of International Global Atmospheric Chemistry (IGAC) and Stratospheric Processes And their Role in Climate (SPARC) under the International Geosphere-Biosphere Project (IGBP) and World Climate Research Program (WCRP). The authors are grateful to the British Atmospheric Data Centre (BADC), which is part of the NERC National Centre for Atmospheric Science (NCAS), for collecting and archiving the ACCMIP data. D. S. thanks James Manners for assistance in setting up the E-S radiation code. GAF, STR and WJC were supported by the Joint DECC and Defra Integrated Climate Programme (GA01101) and the Defra SSNIP air quality contract AQ 0902. GZ acknowledges NIWA HPCF facility and funding from New Zealand Ministry of Science and Innovation. The CESM project is supported by the National Science Foundation and the Office of Science (BER) of the US Department of Energy. The National Center for Atmospheric Research is operated by the University Corporation for Atmospheric Research under sponsorship of the National Science Foundation. The work of DB and PC was funded by the US Dept. of Energy (BER), performed under the auspices of LLNL under Contract DE-AC52-07NA27344, and used the supercomputing resources of NERSC under contract No. DE-AC02-05CH11231. VN and LWH acknowledge efforts of GFDL's Global Atmospheric Model Development Team in the development of the GFDL-AM3 and Modeling Services Group for assistance with data processing. The GEOSCCM work was supported by the NASA Modeling, Analysis and Prediction program, with computing resources provided by NASA's High-End Computing Program through the NASA Advanced Supercomputing Division. The MIROC-CHEM calculations were perfomed on the NIES supercomputer system (NEC SX-8R), and supported by the Environment Research and Technology Development Fund (S-7) of the Ministry of the Environment, Japan. The STOC-HadAM3 work made use of the facilities of HECToR, the UK's national high-performance computing service, which is provided by UoE HPCx Ltd at the University of Edinburgh, Cray Inc and NAG Ltd., and funded by the Office of Science and Technology through EPSRC's High End Computing Programme. The LMDz-OR-INCA simulations were done using computing resources provided by the CCRT/GENCI computer center of the CEA. The CICERO-OsloCTM2 simulations were done within the projects SLAC (Short Lived Atmospheric Components) and EarthClim funded by the Norwegian Research Council. The MOCAGE simulations were supported by Meteo-France and CNRS. Supercomputing time was provided by Meteo-France/DSI supercomputing center. DTS and YHL acknowledge support from the NASA MAP and ACMAP programs. D. P. would like to thank the Canadian Foundation for Climate and Atmospheric Sciences for their long-running support of CMAM development. AC was supported by the SciDAC program of the Dept. of Energy.; Finally, we acknowledge support towards publication costs from the UK Met Office, NOAA, CICERO and NIWA, in the absence of support from Edinburgh University. NR 99 TC 85 Z9 89 U1 6 U2 87 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1680-7316 J9 ATMOS CHEM PHYS JI Atmos. Chem. Phys. PY 2013 VL 13 IS 6 BP 3063 EP 3085 DI 10.5194/acp-13-3063-2013 PG 23 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 117NU UT WOS:000316961000008 ER PT J AU Roberts, YL Pilewskie, P Kindel, BC Feldman, DR Collins, WD AF Roberts, Y. L. Pilewskie, P. Kindel, B. C. Feldman, D. R. Collins, W. D. TI Quantitative comparison of the variability in observed and simulated shortwave reflectance SO ATMOSPHERIC CHEMISTRY AND PHYSICS LA English DT Article ID CLIMATE MODELS; SPECTRA; RADIOMETRY; EARTH AB The Climate Absolute Radiance and Refractivity Observatory (CLARREO) is a climate observation system that has been designed to monitor the Earth's climate with unprecedented absolute radiometric accuracy and SI traceability. Climate Observation System Simulation Experiments (OSSEs) have been generated to simulate CLARREO hyperspectral shortwave imager measurements to help define the measurement characteristics needed for CLARREO to achieve its objectives. To evaluate how well the OSSE-simulated reflectance spectra reproduce the Earth's climate variability at the beginning of the 21st century, we compared the variability of the OSSE reflectance spectra to that of the reflectance spectra measured by the Scanning Imaging Absorption Spectrometer for Atmospheric Cartography (SCIA-MACHY). Principal component analysis (PCA) is a multivariate decomposition technique used to represent and study the variability of hyperspectral radiation measurements. Using PCA, between 99.7% and 99.9% of the total variance the OSSE and SCIAMACHY data sets can be explained by subspaces defined by six principal components (PCs). To quantify how much information is shared between the simulated and observed data sets, we spectrally decomposed the intersection of the two data set subspaces. The results from four cases in 2004 showed that the two data sets share eight (January and October) and seven (April and July) dimensions, which correspond to about 99.9% of the total SCIAMACHY variance for each month. The spectral nature of these shared spaces, understood by examining the transformed eigenvectors calculated from the subspace intersections, exhibit similar physical characteristics to the original PCs calculated from each data set, such as water vapor absorption, vegetation reflectance, and cloud reflectance. C1 [Roberts, Y. L.; Pilewskie, P.] Univ Colorado, Dept Atmospher & Ocean Sci, Boulder, CO 80309 USA. [Roberts, Y. L.; Pilewskie, P.; Kindel, B. C.] Lab Atmospher & Space Sci, Boulder, CO USA. [Roberts, Y. L.] NASA, Langley Res Ctr, Hampton, VA 23665 USA. [Feldman, D. R.; Collins, W. D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Collins, W. D.] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. RP Roberts, YL (reprint author), Univ Colorado, Dept Atmospher & Ocean Sci, Boulder, CO 80309 USA. EM yolanda.l.roberts@nasa.gov RI Feldman, Daniel/N-8703-2013; Collins, William/J-3147-2014; Richards, Amber/K-8203-2015 OI Feldman, Daniel/0000-0003-3365-5233; Collins, William/0000-0002-4463-9848; NR 37 TC 5 Z9 5 U1 0 U2 13 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1680-7316 J9 ATMOS CHEM PHYS JI Atmos. Chem. Phys. PY 2013 VL 13 IS 6 BP 3133 EP 3147 DI 10.5194/acp-13-3133-2013 PG 15 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 117NU UT WOS:000316961000013 ER PT J AU Kulawik, SS Worden, JR Wofsy, SC Biraud, SC Nassar, R Jones, DBA Olsen, ET Jimenez, R Park, S Santoni, GW Daube, BC Pittman, JV Stephens, BB Kort, EA Osterman, GB AF Kulawik, S. S. Worden, J. R. Wofsy, S. C. Biraud, S. C. Nassar, R. Jones, D. B. A. Olsen, E. T. Jimenez, R. Park, S. Santoni, G. W. Daube, B. C. Pittman, J. V. Stephens, B. B. Kort, E. A. Osterman, G. B. CA TES Team TI Comparison of improved Aura Tropospheric Emission Spectrometer CO2 with HIPPO and SGP aircraft profile measurements SO ATMOSPHERIC CHEMISTRY AND PHYSICS LA English DT Article ID CARBON-DIOXIDE; RETRIEVAL ALGORITHM; ERROR ANALYSIS; TES; SATELLITE; SURFACE; ALTITUDE; GASES; SPACE; BIAS AB Thermal infrared radiances from the Troposheric Emission Spectrometer (TES) between 10 and 15 mu m contain significant carbon dioxide (CO2) information, however the CO2 signal must be separated from radiative interference from temperature, surface and cloud parameters, water, and other trace gases. Validation requires data sources spanning the range of TES CO2 sensitivity, which is approximately 2.5 to 12 km with peak sensitivity at about 5 km and the range of TES observations in latitude (40 degrees S to 40 degrees N) and time (2005-2011). We therefore characterize Tropospheric Emission Spectrometer (TES) CO2 version 5 biases and errors through comparisons to ocean and land-based aircraft profiles and to the Carbon Tracker assimilation system. We compare to ocean profiles from the first three Hiaper Pole-to-Pole Observations (HIPPO) campaigns between 40 degrees S and 40 degrees N with measurements between the surface and 14 km and find that TES CO2 estimates capture the seasonal and latitudinal gradients observed by HIPPO CO2 measurements. Actual errors range from 0.8-1.8 ppm, depending on the campaign and pressure level, and are approximately 1.6-2 times larger than the predicted errors. The bias of TES versus HIPPO is within 1 ppm for all pressures and datasets; however, several of the sub-tropical TES CO2 estimates are lower than expected based on the calculated errors. Comparisons to land aircraft profiles from the United States Southern Great Plains (SGP) Atmospheric Radiation Measurement (ARM) between 2005 and 2011 measured form the surface to 5 km to TES CO2 show good agreement with an overall bias of -0.3 ppm to 0.1 ppm and standard deviations of 0.8 to 1.0 ppm at different pressure levels. Extending the SGP aircraft profiles above 5 km using AIRS or CONTRAIL measurements improves comparisons with TES. Comparisons to CarbonTracker (version CT2011) show a persistent spatially dependent bias pattern and comparisons to SGP show a time-dependent bias -0.2 ppm yr(-1). We also find that the predicted sensitivity of the TES CO2 estimates is too high, which results from using a multi-step retrieval for CO2 and temperature. We find that the averaging kernel in the TES product corrected by a pressure-dependent factor accurately reflects the sensitivity of the TES CO2 product. C1 [Kulawik, S. S.; Worden, J. R.; Olsen, E. T.; Kort, E. A.; Osterman, G. B.] CALTECH, Jet Prop Lab, Pasadena, CA 91125 USA. [Wofsy, S. C.; Santoni, G. W.; Daube, B. C.; Pittman, J. V.] Harvard Univ, Sch Engn & Appl Sci, Cambridge, MA 02138 USA. [Wofsy, S. C.; Santoni, G. W.; Daube, B. C.; Pittman, J. V.] Harvard Univ, Dept Earth & Planetary Sci, Cambridge, MA 02138 USA. [Biraud, S. C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Nassar, R.] Environm Canada, Toronto, ON, Canada. [Jones, D. B. A.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Jimenez, R.] Univ Nacl Colombia, Dept Chem & Environm Engn, Air Qual Res Grp, Bogota 111321, DC, Colombia. [Park, S.] Kyungpook Natl Univ, Dept Oceanog, Coll Ecol & Environm Sci, Taegu, South Korea. [Stephens, B. B.] Natl Ctr Atmospher Res, Boulder, CO 80307 USA. RP Kulawik, SS (reprint author), CALTECH, Jet Prop Lab, Pasadena, CA 91125 USA. EM susan.kulawik@jpl.nasa.gov RI Kort, Eric/F-9942-2012; Biraud, Sebastien/M-5267-2013; Stephens, Britton/B-7962-2008; Jones, Dylan/O-2475-2014; OI Kort, Eric/0000-0003-4940-7541; Biraud, Sebastien/0000-0001-7697-933X; Stephens, Britton/0000-0002-1966-6182; Jones, Dylan/0000-0002-1935-3725; Nassar, Ray/0000-0001-6282-1611 FU Office of Biological and Environmental Research of the US Department of Energy as part of the Atmospheric Radiation Measurement Program (ARM), ARM Aerial Facility [DE-AC02-288 05CH11231]; Terrestrial Ecosystem Science Program; National Aeronantics and Space Administration; NASA ACMAP; National Science Foundation (NSF); Scripps Institution of Oceanography; NCAR [ATM-0628575, ATM-0628519, ATM-0628388]; several offices and programs of the National Oceanic and Atmospheric Administration; Atmospheric Composition and Climate Program; Office of Oceanic and Atmospheric Research; Environmental Research Laboratory; NSF FX SGP aircraft measurements were supported by the Office of Biological and Environmental Research of the US Department of Energy under contract No. DE-AC02-288 05CH11231 as part of the Atmospheric Radiation Measurement Program (ARM), ARM Aerial Facility, and Terrestrial Ecosystem Science Program.; Work at the Jet Propulsion Laboratory, California Institute of Technology, was performed under a contract with the National Aeronantics and Space Administration and funded through NASA ACMAP. 2007.; The HIPPO campaign was funded by National Science Foundation (NSF) grants to Harvard University, Scripps Institution of Oceanography, and NCAR (ATM-0628575, ATM-0628519, and ATM-0628388) and by several offices and programs of the National Oceanic and Atmospheric Administration; the Atmospheric Composition and Climate Program, the Office of Oceanic and Atmospheric Research, and the Environmental Research Laboratory. The National Center for Atmospheric Research is sponsored by the NSF. NR 39 TC 8 Z9 8 U1 0 U2 21 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1680-7316 J9 ATMOS CHEM PHYS JI Atmos. Chem. Phys. PY 2013 VL 13 IS 6 BP 3205 EP 3225 DI 10.5194/acp-13-3205-2013 PG 21 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 117NU UT WOS:000316961000018 ER PT J AU Stier, P Schutgens, NAJ Bellouin, N Bian, H Boucher, O Chin, M Ghan, S Huneeus, N Kinne, S Lin, G Ma, X Myhre, G Penner, JE Randles, CA Samset, B Schulz, M Takemura, T Yu, F Yu, H Zhou, C AF Stier, P. Schutgens, N. A. J. Bellouin, N. Bian, H. Boucher, O. Chin, M. Ghan, S. Huneeus, N. Kinne, S. Lin, G. Ma, X. Myhre, G. Penner, J. E. Randles, C. A. Samset, B. Schulz, M. Takemura, T. Yu, F. Yu, H. Zhou, C. TI Host model uncertainties in aerosol radiative forcing estimates: results from the AeroCom Prescribed intercomparison study SO ATMOSPHERIC CHEMISTRY AND PHYSICS LA English DT Article ID GENERAL-CIRCULATION MODEL; PLANETARY ALBEDO; CLIMATE RESPONSE; SATELLITE; SIMULATION; SENSITIVITY; NUCLEATION; SULFATE; SYSTEM; EARTH AB Simulated multi-model "diversity" in aerosol direct radiative forcing estimates is often perceived as a measure of aerosol uncertainty. However, current models used for aerosol radiative forcing calculations vary considerably in model components relevant for forcing calculations and the associated "host-model uncertainties" are generally convoluted with the actual aerosol uncertainty. In this AeroCom Prescribed intercomparison study we systematically isolate and quantify host model uncertainties on aerosol forcing experiments through prescription of identical aerosol radiative properties in twelve participating models. Even with prescribed aerosol radiative properties, simulated clear-sky and all-sky aerosol radiative forcings show significant diversity. For a purely scattering case with globally constant optical depth of 0.2, the global-mean all-sky top-of-atmosphere radiative forcing is -4.47 Wm(-2) and the inter-model standard deviation is 0.55 Wm(-2), corresponding to a relative standard deviation of 12 %. For a case with partially absorbing aerosol with an aerosol optical depth of 0.2 and single scattering albedo of 0.8, the forcing changes to 1.04 Wm(-2), and the standard deviation increases to 1.01 W-2, corresponding to a significant relative standard deviation of 97 %. However, the top-of-atmosphere forcing variability owing to absorption (subtracting the scattering case from the case with scattering and absorption) is low, with absolute (relative) standard deviations of 0.45 Wm(-2) (8 %) clear-sky and 0.62 Wm(-2) (11 %) all-sky. Scaling the forcing standard deviation for a purely scattering case to match the sulfate radiative forcing in the AeroCom Direct Effect experiment demonstrates that host model uncertainties could explain about 36% of the overall sulfate forcing diversity of 0.11 Wm(-2) in the AeroCom Direct Radiative Effect experiment. Host model errors in aerosol radiative forcing are largest in regions of uncertain host model components, such as stratocumulus cloud decks or areas with poorly constrained surface albedos, such as sea ice. Our results demonstrate that host model uncertainties are an important component of aerosol forcing uncertainty that require further attention. C1 [Stier, P.; Schutgens, N. A. J.] Univ Oxford, Dept Phys, Oxford OX1 3PU, England. [Bellouin, N.] Met Off, Hadley Ctr, Exeter, Devon, England. [Bian, H.] Univ Maryland Baltimore Cty, Joint Ctr Earth Syst Technol, Baltimore, MD 21228 USA. [Bian, H.; Chin, M.; Randles, C. A.; Yu, H.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Boucher, O.; Huneeus, N.] UPMC, CNRS, IPSL, Lab Meteorol Dynam, Paris, France. [Ghan, S.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Kinne, S.] Max Planck Inst Meteorol, D-20146 Hamburg, Germany. [Lin, G.; Penner, J. E.; Zhou, C.] Univ Michigan, Dept Atmospher Ocean & Space Sci, Ann Arbor, MI 48109 USA. [Ma, X.; Yu, F.] SUNY Albany, Atmospher Sci Res Ctr, Albany, NY 12222 USA. [Myhre, G.; Samset, B.] CICERO, Oslo, Norway. [Randles, C. A.] Morgan State Univ, GESTAR, Baltimore, MD 21239 USA. [Schulz, M.] Norwegian Meteorol Inst, Oslo, Norway. [Takemura, T.] Kyushu Univ, Appl Mech Res Inst, Fukuoka 8168580, Japan. [Yu, H.] Univ Maryland, Earth Syst Sci Interdisciplinary Ctr, College Pk, MD 20742 USA. RP Stier, P (reprint author), Univ Oxford, Dept Phys, Parks Rd, Oxford OX1 3PU, England. EM philip.stier@physics.ox.ac.uk RI Stier, Philip/B-2258-2008; Takemura, Toshihiko/C-2822-2009; Yu, Hongbin/C-6485-2008; Penner, Joyce/J-1719-2012; Chin, Mian/J-8354-2012; Myhre, Gunnar/A-3598-2008; Schulz, Michael/A-6930-2011; U-ID, Kyushu/C-5291-2016; Ghan, Steven/H-4301-2011; Huneeus, Nicolas/J-4994-2016; ma, xiaoyan/D-2308-2014; Yu, Fangqun/F-3708-2011; Schutgens, Nick/B-2275-2013; Kyushu, RIAM/F-4018-2015 OI Stier, Philip/0000-0002-1191-0128; Huneeus, Nicolas/0000-0002-6214-5518; Bellouin, Nicolas/0000-0003-2109-9559; Zhou, Cheng/0000-0001-9095-2846; Takemura, Toshihiko/0000-0002-2859-6067; Yu, Hongbin/0000-0003-4706-1575; Myhre, Gunnar/0000-0002-4309-476X; Schulz, Michael/0000-0003-4493-4158; Ghan, Steven/0000-0001-8355-8699; Yu, Fangqun/0000-0003-0874-4883; Schutgens, Nick/0000-0001-9805-6384; FU UK Natural Environment Research Council project AEROS on aerosol uncertainties [NE/G006148/1]; US Department of Energy Office of Science Decadal and Regional Climate Prediction using Earth System Models (EaSM) program; DOE by Battelle Memorial Institute [DE-AC06-76RLO 1830]; US National Aeronautics and Space Administration; National Science Foundation; Joint DECC/Defra Met Office Hadley Centre Climate Programme [GA01101]; Funding Program for Next Generation World-Leading Researchers by the Cabinet Office, Government of Japan [GR079] FX This work has been supported by the UK Natural Environment Research Council project AEROS on aerosol uncertainties [NE/G006148/1]. We would like to thank J. Griesfeller (MetNo) for his support with the AeroCom database and Z. Kipling (Oxford) for his helpful comments on the manuscript. S. Ghan was supported by the US Department of Energy Office of Science Decadal and Regional Climate Prediction using Earth System Models (EaSM) program. The Pacific Northwest National Laboratory (PNNL) is operated for the DOE by Battelle Memorial Institute under contract DE-AC06-76RLO 1830. X. Ma and F. Yu were funded by the US National Aeronautics and Space Administration and National Science Foundation. N. Bellouin was supported by the Joint DECC/Defra Met Office Hadley Centre Climate Programme (GA01101). T. Takemura was supported by the Funding Program for Next Generation World-Leading Researchers by the Cabinet Office, Government of Japan (GR079). NR 54 TC 36 Z9 37 U1 4 U2 45 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1680-7316 EI 1680-7324 J9 ATMOS CHEM PHYS JI Atmos. Chem. Phys. PY 2013 VL 13 IS 6 BP 3245 EP 3270 DI 10.5194/acp-13-3245-2013 PG 26 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 117NU UT WOS:000316961000021 ER PT J AU Politz, MC Copeland, MF Pfleger, BF AF Politz, Mark C. Copeland, Matthew F. Pfleger, Brian F. TI Artificial repressors for controlling gene expression in bacteria SO CHEMICAL COMMUNICATIONS LA English DT Article ID TAL EFFECTORS; ESCHERICHIA-COLI; LAC REPRESSOR; PROTEINS; OPERONS AB Transcriptional repression is a common approach to control gene expression in synthetic biology applications. Here, an engineered DNA binding protein based upon a transcription activator-like effector (TALE) scaffold was shown to outperform LacI in blocking transcription from a promoter and to repress expression of a downstream gene in an operon. C1 [Politz, Mark C.; Copeland, Matthew F.; Pfleger, Brian F.] Univ Wisconsin, Dept Chem & Biol Engn, Madison, WI 53706 USA. [Politz, Mark C.; Copeland, Matthew F.; Pfleger, Brian F.] Univ Wisconsin, US DOE, Great Lakes Bioenergy Res Ctr, Madison, WI 53706 USA. RP Pfleger, BF (reprint author), Univ Wisconsin, Dept Chem & Biol Engn, 3629 Engn Hall,1415 Engn Dr, Madison, WI 53706 USA. EM pfleger@wisc.edu FU Wisconsin Alumni Research Foundation; National Science Foundation [EFRI-1240268]; DOE Great Lakes Bioenergy Research Center (DOE BER Office of Sciences) [DE-FC02-07ER64494]; Biotechnology Training Program (NIH) FX This work was funded by the Wisconsin Alumni Research Foundation, the National Science Foundation (EFRI-1240268), and the DOE Great Lakes Bioenergy Research Center (DOE BER Office of Sciences DE-FC02-07ER64494). M. C. P. was supported as a trainee in the Biotechnology Training Program (NIH). NR 17 TC 19 Z9 20 U1 1 U2 32 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1359-7345 J9 CHEM COMMUN JI Chem. Commun. PY 2013 VL 49 IS 39 BP 4325 EP 4327 DI 10.1039/c2cc37107c PG 3 WC Chemistry, Multidisciplinary SC Chemistry GA 130PS UT WOS:000317931500065 PM 23230569 ER PT J AU Li, W Kiran, MSRN Manson, JL Schlueter, JA Thirumurugan, A Ramamurty, U Cheetham, AK AF Li, Wei Kiran, M. S. R. N. Manson, Jamie L. Schlueter, John A. Thirumurugan, A. Ramamurty, U. Cheetham, Anthony K. TI Mechanical properties of a metal-organic framework containing hydrogen-bonded bifluoride linkers SO CHEMICAL COMMUNICATIONS LA English DT Article ID ZEOLITIC IMIDAZOLATE FRAMEWORKS; NANOINDENTATION; ANISOTROPY; CRYSTALS AB We report the mechanical properties of a framework structure, [Cu2F(HF)(HF2)(pyz)(4)][(SbF6)(2)](n) (pyz = pyrazine), in which [Cu(pyz)(2)](2+) layers are pillared by HF2- anions containing the exceptionally strong F-H center dot center dot center dot F hydrogen bonds. Nanoindentation studies on single-crystals clearly demonstrate that such bonds are extremely robust and mechanically comparable with coordination bonds in this system. C1 [Li, Wei; Cheetham, Anthony K.] Univ Cambridge, Dept Mat Sci & Met, Cambridge CB2 3QZ, England. [Kiran, M. S. R. N.; Ramamurty, U.] Indian Inst Sci, Dept Mat Engn, Bangalore 560012, Karnataka, India. [Manson, Jamie L.] Eastern Washington Univ, Dept Chem & Biochem, Cheney, WA 99004 USA. [Schlueter, John A.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Thirumurugan, A.] Indian Inst Sci Educ & Res Thiruvananthapuram, Sch Chem, Thiruvananthapuram 695016, Kerala, India. RP Cheetham, AK (reprint author), Univ Cambridge, Dept Mat Sci & Met, Pembroke St, Cambridge CB2 3QZ, England. EM akc30@cam.ac.uk RI Li, Wei/D-1101-2011; Ramamurty, Upadrasta/E-5623-2011; A, Thirumurugan/A-1825-2010 OI A, Thirumurugan/0000-0001-8469-2718 FU European Research Council; UGC; U.S. Department of Energy Office of Science laboratory [DE-AC02-06CH11357]; U.S. National Science Foundation [DMR-1005825] FX W.L., T.A. and A.K.C. thank the European Research Council for financial support (Advanced Investigator Award to A.K.C.). M.S.R.N.K. thanks the UGC for a Dr D. S. Kothari Post-Doctoral Fellowship. Work at Argonne National Laboratory, a U.S. Department of Energy Office of Science laboratory, was performed under Contract No. DE-AC02-06CH11357. Work at EWU was supported by the U.S. National Science Foundation under grant No. DMR-1005825. NR 31 TC 19 Z9 20 U1 1 U2 72 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1359-7345 J9 CHEM COMMUN JI Chem. Commun. PY 2013 VL 49 IS 40 BP 4471 EP 4473 DI 10.1039/c3cc41357h PG 3 WC Chemistry, Multidisciplinary SC Chemistry GA 130QU UT WOS:000317934700009 PM 23571480 ER PT J AU Guo, BK Ben, T Bi, ZH Veith, GM Sun, XG Qiu, SL Dai, S AF Guo, Bingkun Ben, Teng Bi, Zhonghe Veith, Gabriel M. Sun, Xiao-Guang Qiu, Shilun Dai, Sheng TI Highly dispersed sulfur in a porous aromatic framework as a cathode for lithium-sulfur batteries SO CHEMICAL COMMUNICATIONS LA English DT Article ID IONIC-LIQUID ELECTROLYTE; LI-S BATTERIES; POLYPYRROLE COMPOSITE CATHODES; RECHARGEABLE BATTERIES; CARBON COMPOSITES; PERFORMANCE AB Lithium-sulfur (Li-S) batteries are attractive candidates for transportation applications because of their high energy density (2600 W h kg(-1)). However, Li-S batteries have failed to achieve commercial success, due to the rapid capacity fading with cycling caused mainly by the "shuttle'' phenomenon. Here, we report a feasible approach to mitigate this issue using a porous aromatic framework (PAF) as a hosting substrate in Li-S batteries. As a cathode material, the composite of PAF with sulfur exhibits high capacity and excellent cycling stability in both a sulfone electrolyte, 1.0 M LiPF6-MiPS, and an ionic liquid electrolyte, 0.5 M LiTFSI-MPPY center dot TFSI. C1 [Guo, Bingkun; Bi, Zhonghe; Sun, Xiao-Guang; Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Ben, Teng; Qiu, Shilun] Jilin Univ, Dept Chem, Changchun 130012, Peoples R China. [Veith, Gabriel M.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Dai, Sheng] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. RP Guo, BK (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. EM guob@ornl.gov; sunx@ornl.gov; dais@ornl.gov RI Guo, Bingkun/J-5774-2014; Dai, Sheng/K-8411-2015; Ben, Teng/B-4634-2011 OI Dai, Sheng/0000-0002-8046-3931; Ben, Teng/0000-0002-0847-330X FU U.S. Department of Energy's Office of Basic Energy Science, Division of Materials Sciences and Engineering FX This research was supported by the U.S. Department of Energy's Office of Basic Energy Science, Division of Materials Sciences and Engineering. NR 35 TC 36 Z9 37 U1 16 U2 255 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1359-7345 J9 CHEM COMMUN JI Chem. Commun. PY 2013 VL 49 IS 43 BP 4905 EP 4907 DI 10.1039/c3cc41518j PG 3 WC Chemistry, Multidisciplinary SC Chemistry GA 135VC UT WOS:000318315700010 PM 23604139 ER PT J AU Bejger, C Tian, YH Barker, BJ Boland, KS Scott, BL Batista, ER Kozimor, SA Sessler, JL AF Bejger, Christopher Tian, Yong-Hui Barker, Beau J. Boland, Kevin S. Scott, Brian L. Batista, Enrique R. Kozimor, Stosh A. Sessler, Jonathan L. TI Synthesis and characterization of a tetrathiafulvalene-salphen actinide complex SO DALTON TRANSACTIONS LA English DT Article ID DIMETHYL-SULFOXIDE; N,N-DIMETHYLFORMAMIDE; LUMINESCENT; MOLECULE; LIGAND AB A new tetrathiafulvalene-salphen uranyl complex has been prepared. The system was designed to study the electronic coupling between actinides and a redox active ligand framework. Theoretical and experimental methods - including DFT calculations, single crystal X-ray analysis, cyclic voltammetry, NMR and IR spectroscopies - were used to characterize this new uranyl complex. C1 [Bejger, Christopher; Sessler, Jonathan L.] Univ Texas Austin, Dept Chem & Biochem, Austin, TX 78712 USA. [Bejger, Christopher; Sessler, Jonathan L.] Univ Texas Austin, Inst Cellular & Mol Biol, Austin, TX 78712 USA. [Tian, Yong-Hui; Barker, Beau J.; Boland, Kevin S.; Scott, Brian L.; Batista, Enrique R.; Kozimor, Stosh A.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Sessler, Jonathan L.] Yonsei Univ, Dept Chem, Seoul 120749, South Korea. RP Batista, ER (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM erb@lanl.gov; Stosh@lanl.gov; Sessler@cm.utexas.edu RI Barker, Beau/S-5494-2016; Scott, Brian/D-8995-2017 OI Barker, Beau/0000-0001-6680-6814; Scott, Brian/0000-0003-0468-5396 FU Office of Basic Energy Sciences, U. S. Department of Energy (DOE) [DE-FG02-01ER15186]; Ministry of Education, Science and Technology; Heavy Element Chemistry Program by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy; Glenn T. Seaborg Institute; National Nuclear Security Administration of U.S. Department of Energy [DE-AC52-06NA25396] FX Work at UT Austin was supported by the Office of Basic Energy Sciences, U. S. Department of Energy (DOE) (grant no. DE-FG02-01ER15186 to J.L.S.). J.L.S. also thanks the WCU (World Class University) program of Korea (R32-10217) administered by the National Research Foundation of Korea and funded by the Ministry of Education, Science and Technology. Research at LANL was supported by the Heavy Element Chemistry Program by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy and the Glenn T. Seaborg Institute Graduate and Student Fellowships (CB). LANL is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of U.S. Department of Energy under contract DE-AC52-06NA25396. NR 18 TC 6 Z9 6 U1 2 U2 26 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1477-9226 J9 DALTON T JI Dalton Trans. PY 2013 VL 42 IS 19 BP 6716 EP 6719 DI 10.1039/c3dt50698c PG 4 WC Chemistry, Inorganic & Nuclear SC Chemistry GA 131GV UT WOS:000317981700007 PM 23572119 ER PT J AU Wannarit, N Roubeau, O Youngme, S Teat, SJ Gamez, P AF Wannarit, Nanthawat Roubeau, Olivier Youngme, Sujittra Teat, Simon J. Gamez, Patrick TI Influence of supramolecular bonding contacts on the spin crossover behaviour of iron(II) complexes from 2,2 '-dipyridylamino/s-triazine ligands SO DALTON TRANSACTIONS LA English DT Article ID MEMORY DEVICES; VARIABLE-TEMPERATURE; TRANSITION; LIGHT; COMPOUND; SERIES; SE; PHOTOMAGNETISM; POLYDENTATE; PRESSURE AB Reactions of the related ligands 2-(N,N-bis(2-pyridyl)amino)-4,6-bis(phenoxy)-(1,3,5)triazine (L1) and 2-(N, N-bis(2-pyridyl) amino)-4,6-bis(pentafluorophenoxy)-(1,3,5) triazine (L1(F)) with iron(II) thiocyanate produced two spin-crossover coordination compounds with distinct cooperative behaviours. trans-[Fe-(L1)(2)(NCS)(2)]center dot 2CH(2)Cl(2) (1) displays a very gradual transition centred at T 1/2 = 233 K, characterized by a Delta T-80 (namely the temperature range within which 80% of the transition considered occurs) of 90 K, while that of fluorinated trans-[Fe(L1(F))(2)(NCS)(2)]center dot 2CH(3)CN (3) is significantly more abrupt (and centred at T 1/2 = 238 K), with a Delta T-80 of 50 K, resulting from supramolecular contacts induced by the fluorinated phenol groups. The coordination compound equivalent to 1 with selenocyanate anions, namely trans-[Fe-(L1)(2)(NCSe)(2)]center dot 4CH(2)Cl(2)center dot 4CH(3)OH (2), also exhibits SCO properties centred at T 1/2 = 238 K, but the transition is very gradual (Delta T-80 = 150 K). Light-induced excited spin-state trapping (LIESST) is effective although incomplete for 2 and 3, while it is complete with a T-LIESST of 58 K for 1. C1 [Wannarit, Nanthawat; Gamez, Patrick] Univ Barcelona, Dept Quim Inorgan, QBI, E-08028 Barcelona, Spain. [Roubeau, Olivier] CSIC, Inst Ciencia Mat Aragon ICMA, E-50009 Zaragoza, Spain. [Roubeau, Olivier] Univ Zaragoza, E-50009 Zaragoza, Spain. [Wannarit, Nanthawat; Youngme, Sujittra] Khon Kaen Univ, Dept Chem, Mat Chem Res Unit, Khon Kaen 40002, Thailand. [Wannarit, Nanthawat; Youngme, Sujittra] Khon Kaen Univ, Fac Sci, Ctr Excellence Innovat Chem, Khon Kaen 40002, Thailand. [Teat, Simon J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Gamez, Patrick] Passeig Lluis Co 23, ICREA, Barcelona 08010, Spain. RP Roubeau, O (reprint author), CSIC, Inst Ciencia Mat Aragon ICMA, Plaza San Francisco S-N, E-50009 Zaragoza, Spain. EM patrick.gamez@qi.ub.es RI Gamez, Patrick/B-3610-2012; Roubeau, Olivier/A-6839-2010 OI Gamez, Patrick/0000-0003-2602-9525; Roubeau, Olivier/0000-0003-2095-5843 FU Ministerio de Economia y Competitividad of Spain [CTQ2011-27929-C02-01, MAT2011-24284]; Royal Golden Jubilee Program (RGJ) [PHD/0234/2550]; Khon Kaen University; Office of Science, Office of Basic Energy Sciences of the U. S. Department of Energy [DE-AC02-05CH11231] FX PG acknowledges ICREA (Institucio Catalana de Recerca i Estudis Avancats) and the Ministerio de Economia y Competitividad of Spain (Project CTQ2011-27929-C02-01). NW thanks the Royal Golden Jubilee Program (RGJ, Grant no. PHD/0234/2550) and Khon Kaen University for a research grant. SY acknowledges The Thailand Research Fund, the National Research University Project of Thailand, Office of the Higher Education Commission, through the Advanced Functional Materials Cluster of Khon Kaen University and the Center of Excellence for Innovation in Chemistry (PERCH-CIC), Office of the Higher Education Commission, Ministry of Education. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences of the U. S. Department of Energy under contract no. DE-AC02-05CH11231. OR acknowledges funding from the Ministerio de Economia y Competitividad of Spain (Project MAT2011-24284). NR 64 TC 14 Z9 14 U1 0 U2 32 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1477-9226 J9 DALTON T JI Dalton Trans. PY 2013 VL 42 IS 19 BP 7120 EP 7130 DI 10.1039/c3dt50326g PG 11 WC Chemistry, Inorganic & Nuclear SC Chemistry GA 131GV UT WOS:000317981700051 PM 23525160 ER PT J AU Douglas, EA Zeenberg, D Maeda, M Gila, BP Abernathy, CR Pearton, SJ Ren, F AF Douglas, E. A. Zeenberg, D. Maeda, M. Gila, B. P. Abernathy, C. R. Pearton, S. J. Ren, F. TI Depth-Resolved Cathodoluminescence Spectroscopy Characterization of RF Stressed AlGaN/GaN High Electron Mobility Transistors SO ECS SOLID STATE LETTERS LA English DT Article ID DRAIN BIAS; GAN; HEMTS; RELIABILITY; POWER; PERFORMANCE; DEGRADATION; AMPLIFIERS; SUBSTRATE; OPERATION AB AlGaN/GaN high electron mobility transistors with 0.125 mu m gate length were rf stressed at 10 GHz. Depth resolved cathodoluminescence (CL) was employed to investigate the role of defects in devices that exhibited typical mean time to failure (MTTF) compared to those that suffered from infant mortality. The CL spectra exhibited both laterally and vertically localized defect emission within the channel of devices that failed early, indicating the presence of an increased concentration of V-Ga-based defects within the device. Additionally, residual compressive stress was observed in all devices after electrical stress. (C) 2013 The Electrochemical Society. [DOI: 10.1149/2.002306ssl] All rights reserved. C1 [Douglas, E. A.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Zeenberg, D.; Maeda, M.; Gila, B. P.; Abernathy, C. R.; Pearton, S. J.] Univ Florida, Dept Mat Sci & Engn, Gainesville, FL 32611 USA. [Ren, F.] Univ Florida, Dept Chem Engn, Gainesville, FL 32611 USA. RP Douglas, EA (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM edougla@sandia.gov RI Douglas, Erica/J-3732-2014 OI Douglas, Erica/0000-0003-1873-0223 FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; AFOSR MURI FX Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. The work at UF is supported by an AFOSR MURI monitored by James Hwang. NR 28 TC 1 Z9 1 U1 0 U2 6 PU ELECTROCHEMICAL SOC INC PI PENNINGTON PA 65 SOUTH MAIN STREET, PENNINGTON, NJ 08534 USA SN 2162-8742 J9 ECS SOLID STATE LETT JI ECS Solid State Lett. PY 2013 VL 2 IS 6 BP Q39 EP Q42 DI 10.1149/2.002306ssl PG 4 WC Materials Science, Multidisciplinary; Physics, Applied SC Materials Science; Physics GA 136EP UT WOS:000318344900004 ER PT S AU Fourspring, K Ninkov, Z Heap, S Roberto, M Kim, A AF Fourspring, Kenneth Ninkov, Zoran Heap, Sally Roberto, Massimo Kim, Alex BE Douglass, MR Oden, PI TI Testing of Digital Micromirror Devices for Space-Based Applications SO EMERGING DIGITAL MICROMIRROR DEVICE BASED SYSTEMS AND APPLICATIONS V SE Proceedings of SPIE LA English DT Proceedings Paper CT Conference on Emerging Digital Micromirror Device Based Systems and Applications V CY FEB 05-06, 2013 CL San Francisco, CA SP SPIE, DLP Texas Instruments, VUZIX Corp DE Cryogenic; Digital Micromirror Devices (DMD); low-temperature; MEMS; proton radiation ID MULTIOBJECT SPECTROMETER; PERFORMANCE AB Scientists conceiving future space missions are interested in using DMDs as a multi-object spectrometer (MOS) slit mask. The main uncertainties in utilizing DMDs in a space-based instrument are associated with their operational longevity given the exposure to high levels of proton radiation and their ability to operate at low temperatures. Since a favored orbit is at the second Lagrangian point (L2), it is important to determine how long such Micro-Electrical Mechanical Systems (MEMS) would remain operational in the harsh L2 radiation environment, which primarily consists of solar protons and cosmic rays. To address this uncertainty, we have conducted DMD proton testing at the Lawrence Berkeley National Laboratory (LBNL) 88 '' Cyclotron. Three DMDs were irradiated with high-energy protons (20-50MeV) with energies sufficient to penetrate the DMD package's optical window and interact electrically with the device. After each irradiation step, an optical test procedure was used to validate the operability of each individual mirror on the DMD array. Each DMD was irradiated to a wide range of dosage levels and remained 100% operable up to a total dose of 30 krads. In addition, a few single event upsets were seen during each irradiation dose increment. To determine the minimal operating temperature of the DMDs, we placed a DMD in a liquid nitrogen dewar, and cooled it from room temperature to 130 K. During this test, the DMD was illuminated with a light source and monitored with a CCD camera. Additionally, the temperature was held constant at 173 K for 24 hours to test landing DMD patterns for long periods of time. There was no indication that extended periods of low temperature operation impact the DMD performance. Both of these results point to DMDs as a suitable candidate for future long duration space missions. C1 [Fourspring, Kenneth; Ninkov, Zoran] Rochester Inst Technol, 54 Lomb Mem Dr, Rochester, NY 14623 USA. [Heap, Sally] Space Telescope Sci Inst, Baltimore, MD 21212 USA. [Roberto, Massimo] NASA, Goddard Space Flight Ctr, Code 681, Greenbelt, MD 20771 USA. [Kim, Alex] EO Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Fourspring, K (reprint author), Rochester Inst Technol, 54 Lomb Mem Dr, Rochester, NY 14623 USA. FU NASA Graduate Student Research Program ( GSRP) FX KF would like to thank Sally Heap and NASA Goddard for continued funding through the NASA Graduate Student Research Program ( GSRP). He would also like to thank Peter Hammond of Lightforce Technologies for assistance in designing and manufacturing the dewar parts and Bryan Fodness for support during the irradiation procedure at LBNL. The staff at LBNL's Cyclotron was helpful during our proton testing and we thank them. NR 14 TC 0 Z9 0 U1 1 U2 7 PU SPIE-INT SOC OPTICAL ENGINEERING PI BELLINGHAM PA 1000 20TH ST, PO BOX 10, BELLINGHAM, WA 98227-0010 USA SN 0277-786X BN 978-0-8194-9387-3 J9 PROC SPIE PY 2013 VL 8618 AR 86180B DI 10.1117/12.2006121 PG 10 WC Optics; Physics, Applied SC Optics; Physics GA BET57 UT WOS:000318030300010 ER PT S AU Graff, DL Love, SP AF Graff, David L. Love, Steven P. BE Douglass, MR Oden, PI TI Real-time matched-filter imaging for chemical detection using a DMD-based programmable filter SO EMERGING DIGITAL MICROMIRROR DEVICE BASED SYSTEMS AND APPLICATIONS V SE Proceedings of SPIE LA English DT Proceedings Paper CT Conference on Emerging Digital Micromirror Device Based Systems and Applications V CY FEB 05-06, 2013 CL San Francisco, CA SP SPIE, DLP Texas Instruments, VUZIX Corp DE hyperspectral imaging; Hadamard spectroscopy; spectral matched filters; chemical detection; real-time spectral imaging; micro-mirror array; DLP; DMD ID SPECTROMETER AB Hyperspectral imaging sensors have proven to be powerful tools for highly selective and sensitive chemical detection applications, but have some significant operational drawbacks including a detection time-lag due to the large computational overhead of the matched filter analysis of the resulting data cubes. For applications where only a single chemical is of interest or real-time detection is desired, an intelligently designed multispectral sensor can trade high resolution and continuous spectral coverage for an in-line optical matched filter, enabling snapshot chemical detection with nearly no image processing requirements. Such a system can operate with little loss of performance, greatly reduced data volume, and at a fraction of the cost. We have recently developed a high-speed, high-resolution, programmable spectral filter based on a DLP (R) digital micro-mirror device (DMD) that mimics a conventional band-pass filter by operating on the spectrum without disturbing the underlying image. Our DMD-based filter can independently choose or reject dozens or hundreds of spectral bands and present them simultaneously to an imaging sensor, forming a complete 2D image. With this new technology, even very complicated matched filters can be implemented directly into the optical train of the sensor, producing an image highlighting the target chemical within a spectrally cluttered scene in real-time without further processing. Examples of matched-filter images recorded with our visible-spectrum prototype will be displayed, and extensions to other spectral regions will be discussed. Finally, we will discuss strategies for implementing more sophisticated clutter-suppressing matched filters on the DMD-based system, including schemes that approximate the subtlety of post-processing algorithms by utilizing the DMD's duty-cycle-based gray-scale capability. C1 [Graff, David L.; Love, Steven P.] Los Alamos Natl Lab, Space & Remote Sensing Sci Grp ISR 2, Los Alamos, NM 87544 USA. RP Graff, DL (reprint author), Los Alamos Natl Lab, Space & Remote Sensing Sci Grp ISR 2, Mail Stop B244, Los Alamos, NM 87544 USA. OI Love, Steven/0000-0003-0588-9622 NR 16 TC 2 Z9 2 U1 0 U2 8 PU SPIE-INT SOC OPTICAL ENGINEERING PI BELLINGHAM PA 1000 20TH ST, PO BOX 10, BELLINGHAM, WA 98227-0010 USA SN 0277-786X BN 978-0-8194-9387-3 J9 PROC SPIE PY 2013 VL 8618 AR 86180F DI 10.1117/12.2002694 PG 10 WC Optics; Physics, Applied SC Optics; Physics GA BET57 UT WOS:000318030300014 ER PT S AU Love, SP Graff, DL AF Love, Steven P. Graff, David L. BE Douglass, MR Oden, PI TI Full-frame programmable spectral filters based on micro-mirror arrays SO EMERGING DIGITAL MICROMIRROR DEVICE BASED SYSTEMS AND APPLICATIONS V SE Proceedings of SPIE LA English DT Proceedings Paper CT Conference on Emerging Digital Micromirror Device Based Systems and Applications V CY FEB 05-06, 2013 CL San Francisco, CA SP SPIE, DLP Texas Instruments, VUZIX Corp DE Spectral imager; hyperspectral; DLP; DMD; Hadamard; matched filter; programmable spectral imager AB Rapidly programmable micro-mirror arrays, such as the DLP (R) digital micro-mirror device (DMD), have opened an exciting new arena in spectral imaging: rapidly reprogrammable, high spectral resolution, multi-band spectral filters that perform spectral processing directly in the optical hardware. Such a device is created by placing a DMD at the spectral plane of an imaging spectrometer, and using it as a spectral selector that passes some wavelengths down the optical train to the final image and rejects others. While simple in concept, realizing a truly practical DMD-based spectral filter has proved challenging. Versions described to date have been limited by the intertwining of image position and spectral propagation direction common to most imaging spectrometers, reducing these instruments to line-by-line scanning imagers rather than true spectral cameras that collect entire two-dimensional images at once. Here we report several optical innovations that overcome this limitation and allow us to construct full-frame programmable filters that spectrally manipulate every pixel, simultaneously and without spectral shifts, across a full 2D image. So far, our prototype, which can be programmed either as a matched-filter imager for specific target materials or as a fully hyperspectral multiplexing Hadamard transform imager, has demonstrated over 100 programmable spectral bands while maintaining good spatial image quality. We discuss how diffraction-mediated trades between spatial and spectral resolution determine achievable performance. Finally, we describe methods for dealing with the DLP's 2D diffractive effects, and suggest a simple modification to the DLP that would eliminate their impact for this application. C1 [Love, Steven P.; Graff, David L.] Los Alamos Natl Lab, Space & Remote Sensing Sci Grp ISR 2, Los Alamos, NM 87544 USA. RP Love, SP (reprint author), Los Alamos Natl Lab, Space & Remote Sensing Sci Grp ISR 2, Mail Stop B244, Los Alamos, NM 87544 USA. EM splove@lanl.gov OI Love, Steven/0000-0003-0588-9622 NR 7 TC 2 Z9 2 U1 0 U2 9 PU SPIE-INT SOC OPTICAL ENGINEERING PI BELLINGHAM PA 1000 20TH ST, PO BOX 10, BELLINGHAM, WA 98227-0010 USA SN 0277-786X BN 978-0-8194-9387-3 J9 PROC SPIE PY 2013 VL 8618 AR 86180C DI 10.1117/12.2002659 PG 12 WC Optics; Physics, Applied SC Optics; Physics GA BET57 UT WOS:000318030300011 ER PT S AU Kerfeld, CA Kirilovsky, D AF Kerfeld, Cheryl A. Kirilovsky, Diana BE Chauvat, F CassierChauvat, C TI Structural, Mechanistic and Genomic Insights into OCP-Mediated Photoprotection SO GENOMICS OF CYANOBACTERIA SE Advances in Botanical Research LA English DT Review; Book Chapter ID ORANGE CAROTENOID PROTEIN; SYNECHOCYSTIS PCC 6803; CHLOROPHYLL-BINDING PROTEIN; PHOTOSYSTEM-II; THYLAKOID MEMBRANES; ENERGY-DISSIPATION; STATE TRANSITIONS; BLUE-LIGHT; PHYCOBILISOME FLUORESCENCE; PORPHYRIDIUM-CRUENTUM AB Until relatively recently, photoprotective mechanisms in cyanobacteria were poorly understood. Yet, they play a crucial role in the ecophysiology of cyanobacteria, which inhabit a range of environments, some of them are extreme where stresses such as high salinity, drought and temperature exacerbate the threat of photodamage. This review focuses on the OCP-mediated photoprotective mechanism, which is widespread among cyanobacteria. Mechanistic and structural studies combined with genomic sequence data are painting an increasingly detailed picture of OCP-mediated photoprotection. C1 [Kerfeld, Cheryl A.] US DOE, Joint Genome Inst, Walnut Creek, CA 94598 USA. [Kerfeld, Cheryl A.] Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. [Kirilovsky, Diana] CEA Saclay, UMR8221, Lab Mecanismes Fondamentaux Bioenergie, F-91191 Gif Sur Yvette, France. RP Kerfeld, CA (reprint author), US DOE, Joint Genome Inst, Walnut Creek, CA 94598 USA. EM ckerfeld@lbl.gov NR 81 TC 6 Z9 6 U1 5 U2 27 PU ACADEMIC PRESS LTD-ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL ROAD, LONDON NW1 7DX, ENGLAND SN 0065-2296 BN 978-0-12-394313-2 J9 ADV BOT RES JI Adv. Bot. Res. PY 2013 VL 65 BP 1 EP 26 DI 10.1016/B978-0-12-394313-2.00001-9 PG 26 WC Plant Sciences SC Plant Sciences GA BEL02 UT WOS:000317147100002 ER PT J AU Riley, WJ AF Riley, W. J. TI Using model reduction to predict the soil-surface (COO)-O-18 flux: an example of representing complex biogeochemical dynamics in a computationally efficient manner SO GEOSCIENTIFIC MODEL DEVELOPMENT LA English DT Article ID OXYGEN-ISOTOPE RATIO; ATMOSPHERIC CO2; CARBON-DIOXIDE; ORGANIC-MATTER; 3-DIMENSIONAL SYNTHESIS; CHEMICAL-KINETICS; TALLGRASS PRAIRIE; EDDY COVARIANCE; WATER-VAPOR; DELTA O-18 AB Earth system models (ESMs) must calculate largescale interactions between the land and atmosphere while accurately characterizing fine-scale spatial heterogeneity in water, carbon, and other nutrient dynamics. We present here a high-dimension model representation (HDMR) approach that allows detailed process representation of a coupled carbon and water tracer (the delta O-18 value of the soil-surface CO2 flux (delta F-s)) in a computationally tractable manner. delta F-s depends on the delta O-18 value of soil water, soil moisture and temperature, and soil CO2 production (all of which are depth dependent), and the delta O-18 value of above-surface CO2. We tested the HDMR approach over a growing season in a C-4-dominated pasture using two vertical soil discretizations. The difference between the HDMR approach and the full model solution in the three-month integrated isoflux was less than 0.2% (0.5 mol m(-2) parts per thousand), and the approach is up to 100 times faster than the full numerical solution. This type of model reduction approach allows representation of complex coupled biogeochemical processes in regional and global climate models and can be extended to characterize subgridscale spatial heterogeneity. C1 Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Riley, WJ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Bldg 84-1134,1 Cyclotron Rd, Berkeley, CA 94720 USA. EM wjriley@lbl.gov RI Riley, William/D-3345-2015 OI Riley, William/0000-0002-4615-2304 FU Office of Science, Office of Biological and Environmental Research of the US Department of Energy [DE-AC02-05CH11231] FX This research was supported by the Director, Office of Science, Office of Biological and Environmental Research of the US Department of Energy under Contract No. DE-AC02-05CH11231 as part of their NGEE Arctic and ARM Programs. NR 54 TC 3 Z9 3 U1 1 U2 7 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1991-959X J9 GEOSCI MODEL DEV JI Geosci. Model Dev. PY 2013 VL 6 IS 2 BP 345 EP 352 DI 10.5194/gmd-6-345-2013 PG 8 WC Geosciences, Multidisciplinary SC Geology GA 137LY UT WOS:000318438600005 ER PT J AU Conley, AJ Lamarque, JF Vitt, F Collins, WD Kiehl, J AF Conley, A. J. Lamarque, J. -F. Vitt, F. Collins, W. D. Kiehl, J. TI PORT, a CESM tool for the diagnosis of radiative forcing SO GEOSCIENTIFIC MODEL DEVELOPMENT LA English DT Article ID INTERCOMPARISON PROJECT ACCMIP; CLIMATE MODEL; ATMOSPHERIC CHEMISTRY; ABSORPTION; OZONE AB The Parallel Offline Radiative Transfer (PORT) model is a stand-alone tool, driven by model-generated datasets, that can be used for any radiation calculation that the underlying radiative transfer schemes can perform, such as diagnosing radiative forcing. In its present distribution, PORT isolates the radiation code from the Community Atmosphere Model (CAM4) in the Community Earth System Model (CESM1). The current configuration focuses on CAM4 radiation with the constituents as represented in present-day conditions in CESM1, along with their optical properties. PORT includes an implementation of stratospheric temperature adjustment under the assumption of fixed dynamical heating, which is necessary to compute radiative forcing in addition to the more straightforward instantaneous radiative forcing. PORT can be extended to use radiative constituent distributions from other models or model simulations. Ultimately, PORT can be used with various radiative transfer models. As illustrations of the use of PORT, we perform the computation of radiative forcing from doubling of carbon dioxide, from the change of tropospheric ozone concentration from the year 1850 to 2000, and from present-day aerosols. The radiative forcing from tropospheric ozone (with respect to 1850) generated by a collection of model simulations under the Atmospheric Chemistry and Climate Model Intercomparison Project is found to be 0.34 (with an intermodel standard deviation of 0.07) W m(-2). Present-day aerosol direct forcing (relative to no aerosols) is found to be -1.3 W m(-2). C1 [Conley, A. J.; Lamarque, J. -F.; Vitt, F.; Kiehl, J.] Natl Ctr Atmospher Res, Boulder, CO 80305 USA. [Collins, W. D.] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. [Collins, W. D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Conley, AJ (reprint author), Natl Ctr Atmospher Res, 1850 Table Mesa Dr, Boulder, CO 80305 USA. EM aconley@ucar.edu RI Collins, William/J-3147-2014; Lamarque, Jean-Francois/L-2313-2014 OI Collins, William/0000-0002-4463-9848; Lamarque, Jean-Francois/0000-0002-4225-5074 FU SciDAC project from the Department of Energy; National Science Foundation FX Andrew Conley, Jean-Francois Lamarque, and Francis Vitt were fully or partially supported by the SciDAC project from the Department of Energy. The National Center for Atmospheric Research is operated by the University Corporation for Atmospheric Research under sponsorship of the National Science Foundation. Many thanks to Chuck Bardeen for his helpful comments which improved an earlier version of this paper. NR 17 TC 17 Z9 17 U1 1 U2 15 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1991-959X J9 GEOSCI MODEL DEV JI Geosci. Model Dev. PY 2013 VL 6 IS 2 BP 469 EP 476 DI 10.5194/gmd-6-469-2013 PG 8 WC Geosciences, Multidisciplinary SC Geology GA 137LY UT WOS:000318438600013 ER PT J AU Drewniak, B Song, J Prell, J Kotamarthi, VR Jacob, R AF Drewniak, B. Song, J. Prell, J. Kotamarthi, V. R. Jacob, R. TI Modeling agriculture in the Community Land Model SO GEOSCIENTIFIC MODEL DEVELOPMENT LA English DT Article ID SOIL CARBON DYNAMICS; CROP-CLIMATE MODEL; NITROGEN REMOBILIZATION; TERRESTRIAL CARBON; GLOBAL PATTERNS; MAIZE YIELDS; TILLAGE; WHEAT; SEQUESTRATION; EMISSIONS AB The potential impact of climate change on agriculture is uncertain. In addition, agriculture could influence above-and below-ground carbon storage. Development of models that represent agriculture is necessary to address these impacts. We have developed an approach to integrate agriculture representations for three crop types - maize, soybean, and spring wheat - into the coupled carbon-nitrogen version of the Community Land Model (CLM), to help address these questions. Here we present the new model, CLM-Crop, validated against observations from two AmeriFlux sites in the United States, planted with maize and soybean. Seasonal carbon fluxes compared well with field measurements for soybean, but not as well for maize. CLM-Crop yields were comparable with observations in countries such as the United States, Argentina, and China, although the generality of the crop model and its lack of technology and irrigation made direct comparison difficult. CLM-Crop was compared against the standard CLM3.5, which simulates crops as grass. The comparison showed improvement in gross primary productivity in regions where crops are the dominant vegetation cover. Crop yields and productivity were negatively correlated with temperature and positively correlated with precipitation, in agreement with other modeling studies. In case studies with the new crop model looking at impacts of residue management and planting date on crop yield, we found that increased residue returned to the litter pool increased crop yield, while reduced residue returns resulted in yield decreases. Using climate controls to signal planting date caused different responses in different crops. Maize and soybean had opposite reactions: when low temperature threshold resulted in early planting, maize responded with a loss of yield, but soybean yields increased. Our improvements in CLM demonstrate a new capability in the model - simulating agriculture in a realistic way, complete with fertilizer and residue management practices. Results are encouraging, with improved representation of human influences on the land surface and the potentially resulting climate impacts. C1 [Drewniak, B.; Prell, J.; Kotamarthi, V. R.] Argonne Natl Lab, Div Environm Sci, Argonne, IL 60439 USA. [Song, J.] No Illinois Univ, Dept Geog, De Kalb, IL 60115 USA. [Jacob, R.] Argonne Natl Lab, Div Math & Comp Sci, Argonne, IL 60439 USA. RP Drewniak, B (reprint author), Argonne Natl Lab, Div Environm Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM bbye@anl.gov FU US Department of Energy, Office of Science [DE-AC02-06CH11357]; Office of Science and US Department of Energy [DE-AC02-05CH11231] FX We would like to extend our thanks to Sam Levis for his helpful discussions and guidance with model development. Our gratitude also goes to Bill Sacks for making the Crop Calendar Dataset available for use as model input. The work of Drewniak, Song, Prell, Kotamarthi, and Jacob at Argonne National Laboratory was supported by the US Department of Energy, Office of Science, under contract DE-AC02-06CH11357. Numerical simulations were performed with resources provided by the National Energy Research Scientific Computing Center, supported by the Office of Science and US Department of Energy Contract No. DE-AC02-05CH11231. NR 62 TC 19 Z9 19 U1 5 U2 50 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1991-959X J9 GEOSCI MODEL DEV JI Geosci. Model Dev. PY 2013 VL 6 IS 2 BP 495 EP 515 DI 10.5194/gmd-6-495-2013 PG 21 WC Geosciences, Multidisciplinary SC Geology GA 137LY UT WOS:000318438600015 ER PT J AU Groff, D George, A Sun, N Sathitsuksanoh, N Bokinsky, G Simmons, BA Holmes, BM Keasling, JD AF Groff, Dan George, Anthe Sun, Ning Sathitsuksanoh, Noppadon Bokinsky, Gregory Simmons, Blake A. Holmes, Bradley M. Keasling, Jay D. TI Acid enhanced ionic liquid pretreatment of biomass SO GREEN CHEMISTRY LA English DT Article ID 1-BUTYL-3-METHYLIMIDAZOLIUM CHLORIDE; ENZYMATIC SACCHARIFICATION; CELLULOSE; SWITCHGRASS; BIOFUELS; ETHANOL; SUGARS; RECALCITRANCE; HYDROLYSIS; CHEMICALS AB Acid enhanced ionic liquid pretreatment is a promising method for boosting the yield of sugars produced from purified cellulose. Acid enhancement significantly increases the yields of sugars from the lignocellulosic feedstock switchgrass. The addition of Amberlyst 15, a protic acid resin, to the ionic liquid pretreatment of switchgrass boosted the yield of sugar up to ten times, decreased the amount of cellulase required for saccharification and increased the biocatalytic conversion of switchgrass into free fatty acids 10-fold to 22% of the theoretical yield. C1 [Groff, Dan; George, Anthe; Sun, Ning; Sathitsuksanoh, Noppadon; Bokinsky, Gregory; Simmons, Blake A.; Holmes, Bradley M.; Keasling, Jay D.] Joint BioEnergy Inst, Emeryville, CA USA. [George, Anthe; Simmons, Blake A.; Holmes, Bradley M.] Sandia Natl Labs, Livermore, CA USA. [Keasling, Jay D.] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. [Keasling, Jay D.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. RP Groff, D (reprint author), Joint BioEnergy Inst, Emeryville, CA USA. EM bradley.m.holmes@gmail.com; jdkeasling@lbl.gov RI Sun, Ning/D-6709-2012; Keasling, Jay/J-9162-2012; sathitsuksanoh, noppadon/O-6305-2014; OI Keasling, Jay/0000-0003-4170-6088; sathitsuksanoh, noppadon/0000-0003-1521-9155; Simmons, Blake/0000-0002-1332-1810 FU Office of Science, Office of Biological and Environmental Research, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work conducted by the Joint BioEnergy Institute was supported by the Office of Science, Office of Biological and Environmental Research, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 25 TC 18 Z9 19 U1 3 U2 42 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9262 J9 GREEN CHEM JI Green Chem. PY 2013 VL 15 IS 5 BP 1264 EP 1267 DI 10.1039/c3gc37086k PG 4 WC Chemistry, Multidisciplinary; GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY SC Chemistry; Science & Technology - Other Topics GA 135OB UT WOS:000318296700025 ER PT J AU Tian, WH Samatova, NF AF Tian, Wenhong Samatova, Nagiza F. TI Global Alignment of Pairwise Protein Interaction Networks for Maximal Common Conserved Patterns SO INTERNATIONAL JOURNAL OF GENOMICS LA English DT Article ID WHOLE GENOMES; SPECIFICITY; ANNOTATION; ORTHOLOGS; GENES; YEAST AB A number of tools for the alignment of protein-protein interaction (PPI) networks have laid the foundation for PPI network analysis. Most of alignment tools focus on finding conserved interaction regions across the PPI networks through either local or global mapping of similar sequences. Researchers are still trying to improve the speed, scalability, and accuracy of network alignment. In view of this, we introduce a connected-components based fast algorithm, HopeMap, for network alignment. Observing that the size of true orthologs across species is small comparing to the total number of proteins in all species, we take a different approach based on a precompiled list of homologs identified by KO terms. Applying this approach to S. cerevisiae (yeast) and D. melanogaster (fly), E. coli K12 and S. typhimurium, E. coli K12 and C. crescenttus, we analyze all clusters identified in the alignment. The results are evaluated through up-to-date known gene annotations, gene ontology (GO), and KEGG ortholog groups (KO). Comparing to existing tools, our approach is fast with linear computational cost, highly accurate in terms of KO and GO terms specificity and sensitivity, and can be extended to multiple alignments easily. C1 [Tian, Wenhong] Univ Elect Sci & Technol China, Sch Comp Sci & Engn, Chengdu 611731, Peoples R China. [Samatova, Nagiza F.] Oak Ridge Natl Lab, Dept Comp, Oak Ridge, TN 37831 USA. [Samatova, Nagiza F.] Oak Ridge Natl Lab, Div Math, Oak Ridge, TN 37831 USA. [Samatova, Nagiza F.] N Carolina State Univ, Dept Comp Sci, Raleigh, NC 27696 USA. RP Tian, WH (reprint author), Univ Elect Sci & Technol China, Sch Comp Sci & Engn, Chengdu 611731, Peoples R China. EM tian_wenhong@uestc.edu.cn FU U.S. Department of Energy (DOE), Office of Science; Office of Advanced Scientific Computing Research (ASCR); Office of Biological and Environmental Research (BER); U.S. National Science Foundation (Expeditions in Computing); U.S. DOE [DEAC05-00OR22725] FX The author would like to thank NetworkBLAST and NetworkBLAST-M team, Professor Roded Sharan and Maxim Kalaev et al. for sharing the datasets and helpful communications, and thank Graemlin team (Jason Flannick et al.) from Stanford University for providing PPI network data and useful communications on alignment problems. Also thank journal reviewers for providing helpful suggestions to improve the quality of this paper. The short version of this paper is published in the proceedings of Pacific Symposium on Biocomputing 14, 2009 [33]. This work was supported in part by the U.S. Department of Energy (DOE), Office of Science, the Office of Advanced Scientific Computing Research (ASCR), the Office of Biological and Environmental Research (BER), and the U.S. National Science Foundation (Expeditions in Computing). Oak Ridge National Laboratory is managed by UT-Battelle for the LLC U.S. DOE under Contract no. DEAC05-00OR22725. NR 24 TC 2 Z9 2 U1 0 U2 11 PU HINDAWI PUBLISHING CORPORATION PI NEW YORK PA 410 PARK AVENUE, 15TH FLOOR, #287 PMB, NEW YORK, NY 10022 USA SN 2314-436X J9 INT J GENOMICS JI Int. J. Genomics PY 2013 AR 670623 DI 10.1155/2013/670623 PG 11 WC Biochemistry & Molecular Biology; Biotechnology & Applied Microbiology; Genetics & Heredity SC Biochemistry & Molecular Biology; Biotechnology & Applied Microbiology; Genetics & Heredity GA 135EY UT WOS:000318271900001 ER PT J AU Ramasamy, KK Wang, Y AF Ramasamy, Karthikeyan K. Wang, Yong TI Catalyst activity comparison of alcohols over zeolites SO JOURNAL OF ENERGY CHEMISTRY LA English DT Article DE zeolite; HZSM-5; alcohol conversion; catalyst activity; hydrocarbons ID TO-HYDROCARBONS REACTION; BIOMASS RESOURCES; METHANOL; CONVERSION; H-ZSM-5; ETHANOL; CHEMICALS; CAVITIES; GASOLINE; SAPO-34 AB Alcohol transformation to transportation fuel-range hydrocarbon over HZSM-5 (SiO2/Al2O3 = 30) catalyst was studied at 360 degrees C and 300 psig. Product distributions and catalyst life were compared between methanol, ethanol, 1-propanol and 1-butanol as a feed. The catalyst life for 1-propanol and 1-butanol was more than double compared with that for methanol and ethanol. For all the alcohols studied, the product distributions (classified to paraffin, olefin, naphthene, aromatic and naphthalene compounds) varied with time on stream (TOS). At 24 h TOS, liquid product from 1-propanol and 1-butanol transformation primarily contains higher olefin compounds. The alcohol transformation process to higher hydrocarbon involves a complex set of reaction pathways such as dehydration, oligomerization, dehydrocyclization and hydrogenation. Compared with ethylene generated from methanol and ethanol, oligomerization of propylene and butylene has a lower activation energy and can readily take place on weaker acidic sites. On the other hand, dehydrocyclization of the oligomerized products of propylene and butylene to form the cyclic compounds requires the sites with stronger acid strength. Combination of the above mentioned reasons are the primary reasons for olefin rich product generated in the later stage of the time on stream and for the extended catalyst life time for 1-propanol and 1-butanol compared with methanol and ethanol conversion over HZSM-5. C1 [Ramasamy, Karthikeyan K.; Wang, Yong] Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99354 USA. [Ramasamy, Karthikeyan K.; Wang, Yong] Washington State Univ, Voiland Sch Chem Engn & Bioengn, Pullman, WA 99163 USA. RP Wang, Y (reprint author), Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99354 USA. EM karthi@pnnl.gov; yong.wang@pnnl.gov RI Ramasamy, karthikeyan/C-3258-2014; Ramasamy, karthikeyan/H-9981-2014 FU Pacific Northwest National Laboratory; U. S. Department of Energy [DE-AC05-76RL01830] FX This work was supported by the Pacific Northwest National Laboratory's Laboratory Directed Research and Development Funding. Pacific Northwest National Laboratory is operated by Battelle Memorial Institute for the U. S. Department of Energy under Contract No. DE-AC05-76RL01830. NR 23 TC 15 Z9 15 U1 3 U2 78 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 2095-4956 J9 J ENERGY CHEM JI J. Energy Chem. PD JAN PY 2013 VL 22 IS 1 BP 65 EP 71 PG 7 WC Chemistry, Applied; Chemistry, Physical; Energy & Fuels; Engineering, Chemical SC Chemistry; Energy & Fuels; Engineering GA 132EM UT WOS:000318050700009 ER PT J AU Kaur, M Johnson, A Tian, GX Jiang, WL Rao, LF Paszczynski, A Qiang, Y AF Kaur, Maninder Johnson, Andrew Tian, Guoxin Jiang, Weilin Rao, Linfeng Paszczynski, Andrzej Qiang, You TI Separation nanotechnology of diethylenetriaminepentaacetic acid bonded magnetic nanoparticles for spent nuclear fuel SO NANO ENERGY LA English DT Article DE Magnetic nanoparticles; Functionalization; Actinides; Sorption; Magnetic separation; Hydrodynamic size ID ASSISTED CHEMICAL-SEPARATION; FISSION-PRODUCT; PARTICLES; EXTRACTANTS; PLUTONIUM; SILICA AB A nanomagnetic separation method based on diethylenetriaminepentaacetic acid (DTPA) conjugated with magnetic nanoparticles (MNPs) is studied for application in spent nuclear fuel separation. The high affinity of DTPA towards actinides aids in separation from the highly acidic medium of nuclear waste. The solubility and magnetization of particles at tow pH is protected by encapsulating them in silica. Surface functionalization of silica coated particles with polyamines enhances the loading capacity of the chelator on MNPs. The particles were characterized before and after surface modification using different characterizing tools. The uptake behavior of Am(III), Pu(IV), U(VI), and Np(V) from 0.1 M NaNO3 solution was determined. The sorption results show the strong affinity of DTPA towards Am(III) and Pu(IV) by extracting 97% and 80% of actinides, respectively. The high removal efficiency of actinides make the chelator conjugated MNPs an effective method for spent nuclear fuel separation. (C) 2012 Elsevier Ltd. All rights reserved. C1 [Kaur, Maninder; Qiang, You] Univ Idaho, Dept Phys, Moscow, ID 83844 USA. [Kaur, Maninder; Qiang, You] Univ Idaho, Environm Sci Program, Moscow, ID 83844 USA. [Johnson, Andrew; Paszczynski, Andrzej] Univ Idaho, Sch Food Sci, Moscow, ID 83844 USA. [Tian, Guoxin; Rao, Linfeng] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Jiang, Weilin] Pacific NW Natl Lab, Richland, WA 99352 USA. [Qiang, You] Ctr Adv Energy Studies, Idaho Falls, ID 83401 USA. RP Qiang, Y (reprint author), Univ Idaho, Dept Phys, Moscow, ID 83844 USA. EM Weilin.Jiang@pnnl.gov; andrzej@uidaho.edu; youqiang@uidaho.edu OI Jiang, Weilin/0000-0001-8302-8313 FU U.S. Department of Energy (DOE) [DE-FC07-08ID14926]; U.S. DOE, Office of Nuclear Energy, the Fuel Research and Development Program [DE-AC02-05CH11231]; DOE BES FX This study was supported by U.S. Department of Energy (DOE) under Contract DE-FC07-08ID14926 (Conjugates of Actinide-Chelator-Magnetic Nanoparticles for Used Fuel Separation Technology). The actinide sorption studies were supported by U.S. DOE, Office of Nuclear Energy, the Fuel Research and Development Program under Contract no. DE-AC02-05CH11231 at Lawrence Berkeley National Laboratory. A portion of the research was conducted in the Environmental Molecular Sciences Laboratory (EMSL), a DOE user facility operated by Battelle for DOE Office of Biological and Environmental Research under Proposal ID# 39391 for TEM, XRD and DLS, and under Proposal ID# 44713 for HIM. Jiang was supported in part by DOE BES. NR 30 TC 14 Z9 14 U1 2 U2 26 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 2211-2855 J9 NANO ENERGY JI Nano Energy PD JAN PY 2013 VL 2 IS 1 BP 124 EP 132 DI 10.1016/j.nanoen.2012.08.005 PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 132EK UT WOS:000318050500018 ER PT J AU Modestino, MA Diaz-Botia, CA Haussener, S Gomez-Sjoberg, R Ager, JW Segalman, RA AF Modestino, Miguel A. Diaz-Botia, Camilo A. Haussener, Sophia Gomez-Sjoberg, Rafael Ager, Joel W. Segalman, Rachel A. TI Integrated microfluidic test-bed for energy conversion devices SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID REDOX-FLOW BATTERIES; HYDROGEN-PRODUCTION; FUEL-CELL; LAMINAR-FLOW; WATER; SYSTEMS; CATALYSTS; STORAGE; ACID AB Energy conversion devices require the parallel functionality of a variety of components for efficient operation. We present a versatile microfluidic test-bed for facile testing of integrated catalysis and mass transport components for energy conversion via water electrolysis. This system can be readily extended to solar-fuels generators and fuel-cell devices. C1 [Modestino, Miguel A.; Segalman, Rachel A.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Modestino, Miguel A.; Ager, Joel W.; Segalman, Rachel A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Modestino, Miguel A.; Haussener, Sophia; Ager, Joel W.; Segalman, Rachel A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA. [Diaz-Botia, Camilo A.; Gomez-Sjoberg, Rafael] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Engn, Berkeley, CA 94720 USA. [Haussener, Sophia] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Haussener, Sophia] Ecole Polytech Fed Lausanne, Inst Engn Mech, CH-1015 Lausanne, Switzerland. RP Ager, JW (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM jwager@lbl.gov; segalman@berkeley.edu OI Ager, Joel/0000-0001-9334-9751; Segalman, Rachel/0000-0002-4292-5103 FU Office of Science of the U.S. Department of Energy [DE-SC0004993]; Engineering Division at Lawrence Berkeley National Laboratory [DE-AC02-05CH11231] FX This material is based upon work performed by the Joint Center for Artificial Photosynthesis, a DOE Energy Innovation Hub, as follows: the electrochemical and transport characterization was supported through the Office of Science of the U.S. Department of Energy under Award no. DE-SC0004993; the development of the microfluidic devices was supported by the Engineering Division at Lawrence Berkeley National Laboratory under contract number DE-AC02-05CH11231. The authors thank Jeff Beeman for help with catalyst deposition, as well as Tyler Matthews, Kenneth Lee, Karl Walczak, and Carl Koval for helpful discussions and experimental assistance. NR 25 TC 9 Z9 9 U1 0 U2 25 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PY 2013 VL 15 IS 19 BP 7050 EP 7054 DI 10.1039/c3cp51302e PG 5 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 131GK UT WOS:000317980600007 PM 23579859 ER PT J AU Summerscales, OT Gordon, JC AF Summerscales, Owen T. Gordon, John C. TI Complexes containing multiple bonding interactions between lanthanoid elements and main-group fragments SO RSC ADVANCES LA English DT Review ID C-H ACTIVATION; HETEROCYCLIC CARBENE COMPLEXES; EARTH METHYLIDENE COMPLEXES; ALUMINUM-CARBON CLUSTER; BASE INDUCED REDUCTIONS; TERMINAL IMIDO COMPLEX; TRANSITION-METAL; STRUCTURAL-CHARACTERIZATION; CRYSTAL-STRUCTURES; PHOSPHORANEIMINATO COMPLEXES AB In this review we detail recent developments in the synthesis of lanthanoid complexes (group III and lanthanide elements) containing multiple bonding interactions with tetrel, pnictogen and chalcogen main group elements. C1 [Summerscales, Owen T.; Gordon, John C.] Los Alamos Natl Lab, Div Chem, Los Alamos, NM 87545 USA. RP Summerscales, OT (reprint author), Los Alamos Natl Lab, Div Chem, MS J582, Los Alamos, NM 87545 USA. EM jgordon@lanl.gov FU Los Alamos National Laboratory FX OTS gratefully acknowledges receipt of a Director's Postdoctoral Fellowship at Los Alamos National Laboratory. NR 104 TC 35 Z9 35 U1 7 U2 51 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2046-2069 J9 RSC ADV JI RSC Adv. PY 2013 VL 3 IS 19 BP 6682 EP 6692 DI 10.1039/c3ra23151h PG 11 WC Chemistry, Multidisciplinary SC Chemistry GA 130PE UT WOS:000317929800001 ER PT S AU Sheik-Bahae, M Ghasemkhani, M Albrecht, AR Seletskiy, DV Cederberg, JG Melgaard, SD AF Sheik-Bahae, Mansoor Ghasemkhani, Mohammad Albrecht, Alexander R. Seletskiy, Denis V. Cederberg, Jeffrey G. Melgaard, Seth D. BE Hastie, JE TI Work at UNM was supported by DARPA GRANT 10669320, AFOSR ( STTR program), and AFRL/ RV University Small Grant. VECSEL growth was supported by Sandia's Laboratory Directed Research and Development Office. Sandia National Laboratories is a multi- program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U. S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. D. V. S acknowledges support by the National Science Foundation under Award No. 1160764. SO VERTICAL EXTERNAL CAVITY SURFACE EMITTING LASERS (VECSELS) III SE Proceedings of SPIE LA English DT Proceedings Paper CT Conference on Vertical External Cavity Surface Emitting Lasers (VECSELs) III CY FEB 03-05, 2013 CL San Francisco, CA SP SPIE, Coherent, Inc DE Optical refrigeration; laser cooling of solids; VECSEL AB Laser cooling of solids to 148 K has been demonstrated in a Yb:YLF crystal using intracavity absorption enhancement in an InGaAs MQW VECSEL at 1020 nm. This is the lowest temperature achieved in the intracavity geometry to date and presents a significant advancement towards an all-solid-state compact cryocooler. C1 [Sheik-Bahae, Mansoor; Ghasemkhani, Mohammad; Albrecht, Alexander R.; Melgaard, Seth D.] Univ New Mexico, Dept Phys & Astron, 1919 Lomas Blvd NE, Albuquerque, NM 87131 USA. [Seletskiy, Denis V.] Univ Konstanz, Dept Phys, Ctr Appl Photon, Constance, Germany. [Cederberg, Jeffrey G.] Sandia Natl Labs, Albuquerque, NM 94550 USA. RP Sheik-Bahae, M (reprint author), Univ New Mexico, Dept Phys & Astron, 1919 Lomas Blvd NE, Albuquerque, NM 87131 USA. EM msb@unm.edu FU DARPA [10669320]; AFOSR; STTR; AFRL/ RV; VECSEL; Sandia National Laboratories is a multi- program laboratory managed and operated by Sandia Corporation; U. S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; National Science Foundation [1160764] FX Work at UNM was supported by DARPA GRANT 10669320, AFOSR ( STTR program), and AFRL/ RV University Small Grant. VECSEL growth was supported by Sandia's Laboratory Directed Research and Development Office. Sandia National Laboratories is a multi- program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U. S. Department of Energy's National Nuclear Security Administration under contract DE- AC04-94AL85000. D. V. S acknowledges support by the National Science Foundation under Award No. 1160764. NR 8 TC 1 Z9 1 U1 3 U2 3 PU SPIE-INT SOC OPTICAL ENGINEERING PI BELLINGHAM PA 1000 20TH ST, PO BOX 10, BELLINGHAM, WA 98227-0010 USA SN 0277-786X BN 978-0-8194-9375-0 J9 PROC SPIE PY 2013 VL 8606 AR 86060A DI 10.1117/12.2003561 PG 6 WC Optics; Physics, Applied SC Optics; Physics GA BET49 UT WOS:000318027500007 ER PT S AU Hahn, HA AF Hahn, Heidi Ann BE Paredis, CJJ Bishop, C Bodner, D TI The conundrum of verification and validation of social science-based models SO 2013 CONFERENCE ON SYSTEMS ENGINEERING RESEARCH SE Procedia Computer Science LA English DT Proceedings Paper CT 11th Annual Conference on Systems Engineering Research (CSER) CY MAR 19-22, 2013 CL Georgia Inst Technol, Atlanta, GA SP Georgia Res Tech Inst, Intercax, IBM Res HO Georgia Inst Technol DE Verification and validation; social science-based models AB In the systems engineering lexicon, definitions for the terms "verification" and "validation" are settled; consistent with the definitions promulgated by the Department of Defense (DoD) [1]; and quite distinct from one another. Verification confirms that all elements of the system meet technical requirements (the product was built right). Validation confirms that the realized system complies with stakeholder requirements (the right system was built). The distinction becomes blurred, however, when one considers verification and validation (V&V) of social science-based models and simulations. Unlike physics-based models, the theoretical underpinnings of Human, Social, Cultural, and Behavioral (HSCB) or other social science models are not readily verified through observation of real-world events or empirical testing. As a result, the theoretical claims on which the models are built are often contested. As noted by Lustick and Tubin [2], when experts do not agree on what the right thing is, determining that the model is built right cannot be separated from tests of whether the right thing has been built. Because systems engineers may encounter social-science based models either in the context of system design or verification, where they may be used as substitutes for human operators or users, or when they are components of a physical system, as is the case when HSCB models are embedded into enhanced persistent surveillance systems for military or intelligence applications, it is important that they understand the limitations and controversies surrounding V&V of these types of models. In this paper, the literature on V&V of models is reviewed, with an emphasis on social science models and some recently developed constructs for their verification and validation. Future directions for social science-based model development and V&V are briefly outlined. (C) 2013 The Authors. Published by Elsevier B. V. Selection and/or peer-review under responsibility of Georgia Institute of Technology C1 Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Hahn, HA (reprint author), Los Alamos Natl Lab, POB 1663 MS F696, Los Alamos, NM 87545 USA. EM Hahn@lanl.gov NR 15 TC 3 Z9 3 U1 0 U2 0 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA SARA BURGERHARTSTRAAT 25, PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 1877-0509 J9 PROCEDIA COMPUT SCI PY 2013 VL 16 BP 878 EP 887 DI 10.1016/j.procs.2013.01.092 PG 10 WC Computer Science, Interdisciplinary Applications; Engineering, Industrial; Operations Research & Management Science SC Computer Science; Engineering; Operations Research & Management Science GA BEL52 UT WOS:000317222600092 ER PT J AU Groenewold, GS Scott, JR Lee, ED Lammert, SA AF Groenewold, Gary S. Scott, Jill R. Lee, Edgar D. Lammert, Stephen A. TI Rapid analysis of organophosphonate compounds recovered from vinyl floor tile using vacuum extraction coupled with a fast-duty cycle GC/MS SO ANALYTICAL METHODS LA English DT Article ID SOLID-PHASE MICROEXTRACTION; VOLATILE ORGANIC-COMPOUNDS; DESORPTION ELECTROSPRAY-IONIZATION; CHROMATOGRAPHY-MASS-SPECTROMETRY; CHEMICAL WARFARE AGENTS; PORTABLE GAS-CHROMATOGRAPHY; EMISSION CELL FLEC; DEGRADATION-PRODUCTS; ATMOSPHERIC-PRESSURE; THERMAL-DESORPTION AB In a terrorist event or industrial accident, environmental toxins will be inhomogeneously distributed on surfaces. A field vacuum extractor (FVE) can be used to sample contamination on fixed surfaces in a non-destructive fashion, but application to heterogeneously contaminated environments tends to be limited by the sampling time and time required for analysis, which is similar to 15 to 30 min for a laboratory gas chromatograph/mass spectrometer (GC/MS). In the present study, FVE surface sampling was combined with a portable, fast-duty cycle GC/MS that enables analysis of a surface sample approximately every 3 minutes. Employing multiple FVE devices enables rapid measurement of many samples as might be required for characterizing contamination that is inhomogeneously distributed in a release environment. The FVE utilizes solid phase microextraction (SPME) fibers to sorb volatilized compounds from an evacuated headspace enclosed over the surface to be sampled (vinyl floor tile in the present study), over the course of a 30 min sampling time. Recovery of organophosphonate compounds in quantities sufficient to enable identification was achieved sampling floor tile exposed to as little as 30 ng. The amount detected was found to increase in a linear fashion with quantity applied to the floor tile, over three orders of magnitude. Carboxen-polydimethylsiloxane (PDMS) was used as the SPME sorbent phase and was sufficiently robust for multiple sampling and analysis cycles. The carboxen-PDMS retained 2-5% of the organophosphonate compounds after the initial GC/MS analysis, and this fraction could be readily measured in a subsequent re-analysis of the same sample. The re-analysis showed identifiable quantities of the organophosphonate compounds in all experiments except those with the lowest exposure quantities. Thus, once-analyzed carboxen-PDMS fibers may be archived for re-analysis at a later date if desired. C1 [Groenewold, Gary S.; Scott, Jill R.] Idaho Natl Lab, Idaho Falls, ID USA. [Lee, Edgar D.; Lammert, Stephen A.] Torion Technol Inc, Amer Fork, UT USA. RP Scott, JR (reprint author), Idaho Natl Lab, Idaho Falls, ID USA. EM jill.scott@inl.gov; ed.lee@torion.com FU Department of Homeland Security, Office of Research and Development; DOE Idaho Operations Office [DE-AC07-05ID14517] FX This research was funded by the Department of Homeland Security, Office of Research and Development and was performed at the Idaho National Laboratory under DOE Idaho Operations Office Contract DE-AC07-05ID14517. NR 60 TC 3 Z9 3 U1 0 U2 26 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1759-9660 J9 ANAL METHODS-UK JI Anal. Methods PY 2013 VL 5 IS 9 BP 2227 EP 2236 DI 10.1039/c3ay26280d PG 10 WC Chemistry, Analytical; Food Science & Technology; Spectroscopy SC Chemistry; Food Science & Technology; Spectroscopy GA 127HX UT WOS:000317690200011 ER PT J AU Doi, K Togano, E Xantheas, SS Nakanishi, R Nagata, T Ebata, T Inokuchi, Y AF Doi, Keisuke Togano, Eijiro Xantheas, Sotiris S. Nakanishi, Ryuzo Nagata, Takashi Ebata, Takayuki Inokuchi, Yoshiya TI Microhydration Effects on the Intermediates of the S(N)2 Reaction of Iodide Anion with Methyl Iodide SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE halides; IR spectroscopy; S(N)2 reactions; solvent effects ID NUCLEOPHILIC DISPLACEMENT-REACTIONS; GAS-PHASE MEASUREMENTS; STEPWISE SOLVATION; SN2 REACTION; KINETICS; CL; TEMPERATURE; SIMULATIONS; SOLVENT; SURFACE C1 [Doi, Keisuke; Togano, Eijiro; Ebata, Takayuki; Inokuchi, Yoshiya] Hiroshima Univ, Grad Sch Sci, Dept Chem, Higashihiroshima 7398526, Japan. [Xantheas, Sotiris S.] Pacific NW Natl Lab, Chem & Mat Sci Div, Richland, WA 99352 USA. [Nakanishi, Ryuzo; Nagata, Takashi] Univ Tokyo, Grad Sch Arts & Sci, Dept Basic Sci, Tokyo 1538902, Japan. RP Inokuchi, Y (reprint author), Hiroshima Univ, Grad Sch Sci, Dept Chem, Higashihiroshima 7398526, Japan. EM y-inokuchi@hiroshima-u.ac.jp RI Inokuchi, Yoshiya/D-4681-2013; Xantheas, Sotiris/L-1239-2015; OI Inokuchi, Yoshiya/0000-0001-7959-5315; Xantheas, Sotiris/0000-0002-6303-1037 FU Ministry of Education, Culture, Sports, Science, and Technology (MEXT) of Japan [21350016]; US Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences Biosciences FX This work is supported by Grant-in-Aids (21350016) for Scientific Research from the Ministry of Education, Culture, Sports, Science, and Technology (MEXT) of Japan. S.S.X. acknowledges support from the US Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences & Biosciences. Pacific Northwest National Laboratory (PNNL) is a multiprogram national laboratory operated for the DOE by Battelle. NR 22 TC 10 Z9 10 U1 0 U2 27 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PY 2013 VL 52 IS 16 BP 4380 EP 4383 DI 10.1002/anie.201207697 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA 126KW UT WOS:000317615000010 PM 23361998 ER PT J AU Lin, LC Kim, J Kong, XQ Scott, E McDonald, TM Long, JR Reimer, JA Smit, B AF Lin, Li-Chiang Kim, Jihan Kong, Xueqian Scott, Eric McDonald, Thomas M. Long, Jeffrey R. Reimer, Jeffrey A. Smit, Berend TI Understanding CO2 Dynamics in Metal-Organic Frameworks with Open Metal Sites SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE carbon dioxide capture; chemical shift anisotropy; CO2 dynamics; metal-organic frameworks ID CARBON-DIOXIDE CAPTURE; ADSORPTION; SIMULATIONS; BINDING; N-2 C1 [Lin, Li-Chiang; Kong, Xueqian; Scott, Eric; Reimer, Jeffrey A.; Smit, Berend] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Kim, Jihan; McDonald, Thomas M.; Long, Jeffrey R.; Smit, Berend] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA USA. [Kong, Xueqian; Reimer, Jeffrey A.] Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA USA. [McDonald, Thomas M.; Long, Jeffrey R.; Smit, Berend] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. RP Lin, LC (reprint author), Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. EM lichianglin@berkeley.edu RI Smit, Berend/B-7580-2009; EFRC, CGS/I-6680-2012; Kim, Jihan/H-8002-2013; Lin, Li-Chiang/J-8120-2014; Stangl, Kristin/D-1502-2015; OI Smit, Berend/0000-0003-4653-8562; Lin, Li-Chiang/0000-0002-2821-9501 FU Center for Gas Separations Relevant to Clean Energy Technologies, an Energy Frontier Research Center; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001015] FX This research was supported through the Center for Gas Separations Relevant to Clean Energy Technologies, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under award DE-SC0001015. NR 29 TC 68 Z9 68 U1 11 U2 161 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PY 2013 VL 52 IS 16 BP 4410 EP 4413 DI 10.1002/anie.201300446 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA 126KW UT WOS:000317615000017 PM 23554332 ER PT S AU Gilles, D Turck-Chieze, S Busquet, M Thais, F Loisel, G Piau, L Ducret, JE Blenski, T Poirier, M Blancard, C Cosse, P Faussurier, G Gilleron, F Pain, JC Guzik, JA Kilcrease, DP Magee, NH Harris, J Bastiani-Ceccotti, S Delahaye, F Zeippen, CJ AF Gilles, D. Turck-Chieze, S. Busquet, M. Thais, F. Loisel, G. Piau, L. Ducret, J. E. Blenski, T. Poirier, M. Blancard, C. Cosse, P. Faussurier, G. Gilleron, F. Pain, J. C. Guzik, J. A. Kilcrease, D. P. Magee, N. H. Harris, J. Bastiani-Ceccotti, S. Delahaye, F. Zeippen, C. J. BE Stehle, C Joblin, C DHendecourt, L TI INTERACTION OF CONFIGURATION IN SPECTRAL OPACITY CALCULATIONS FOR STELLAR PHYSICS SO ECLA: EUROPEAN CONFERENCE ON LABORATORY ASTROPHYSICS SE EAS Publications Series LA English DT Proceedings Paper CT ECLA: European Conference on Laboratory Astrophysics CY SEP 26-30, 2011 CL Paris, FRANCE SP Minist Enseignement Super Rech, CNRS, Programme Natl Phys & Chim, Observ Paris, Univ Pierre & Marie Curie, Univ Cergy Pontolse, Univ Paris Sud, Ctr Natl Etudes Spatiales, Commissariat Energie Atom, Inst Astrophys Paris, Inst Rech Astrophys & Plantetol, Lab Etude Matiere & Env Astrophys, Soc Bruker, Ville Paris ID LOCAL-DENSITY APPROXIMATION; CODE; PLASMAS AB We discuss the role of Configuration Interaction (CI) and the influence of the number of configurations taken into account in the calculations of nickel and iron spectral opacities provided by the OPAC international collaboration, including statistical approaches (SCO, CASSANDRA, STA), detailed accounting (OPAS, LEDCOP, OP, HULLAC-v9) or hybrid method (SCO-RCG). Opacity calculations are presented for a temperature T of 27.3 eV and a density of 3.4 mg/cm(3), conditions relevant for pulsating stellar envelopes. C1 [Gilles, D.; Turck-Chieze, S.; Piau, L.; Ducret, J. E.] CE Saclay, SAp IRFU DSM, F-91191 Gif Sur Yvette, France. [Busquet, M.] ARTEP Ellicott City, Ellicott City, MD 21042 USA. [Thais, F.; Blenski, T.; Poirier, M.] CEA, IRAMIS, SPAM, F-91191 Gif Sur Yvette, France. [Loisel, G.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Blancard, C.; Cosse, P.; Faussurier, G.; Gilleron, F.; Pain, J. C.] CEA, DAM, DIF, F-91297 Arpajon, France. [Guzik, J. A.; Kilcrease, D. P.; Magee, N. H.] LANL, Div Theoret, Los Alamos, NM 87545 USA. [Harris, J.] AWE Reading Berkshire, Aldermaston RG7 4PR, England. [Bastiani-Ceccotti, S.] Ecole Polytechn, LULI, F-91128 Palaiseau, France. [Delahaye, F.; Zeippen, C. J.] CNRS, LERMA, UMR 8112, Observatoire Paris,UPMC, 5 Pl J Janssen, F-92195 Meudon, France. RP Gilles, D (reprint author), CE Saclay, SAp IRFU DSM, F-91191 Gif Sur Yvette, France. OI Pain, Jean-Christophe/0000-0002-7825-1315; Kilcrease, David/0000-0002-2319-5934 NR 14 TC 4 Z9 4 U1 0 U2 4 PU E D P SCIENCES PI CEDEX A PA 17 AVE DU HOGGAR PARC D ACTIVITES COUTABOEUF BP 112, F-91944 CEDEX A, FRANCE SN 1633-4760 BN 978-2-7598-0941-7 J9 EAS PUBLICATIONS PY 2013 VL 58 BP 51 EP + DI 10.1051/eas/1258007 PG 2 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA BEP63 UT WOS:000317632700007 ER PT J AU Al-Naib, I Singh, R Shalaby, M Ozaki, T Morandotti, R AF Al-Naib, Ibraheem Singh, Ranjan Shalaby, Mostafa Ozaki, Tsuneyuki Morandotti, Roberto TI Enhanced Q-factor in Optimally Coupled Macrocell THz Metamaterials: Effect of Spatial Arrangement SO IEEE JOURNAL OF SELECTED TOPICS IN QUANTUM ELECTRONICS LA English DT Article DE Coupling effects; Fano resonance; LC resonance; metamaterials (MTMs); periodic structures; quality factor (Q-factor); spatial arrangement; terahertz (THz) spectroscopy ID SPLIT-RING RESONATORS; TERAHERTZ METAMATERIALS; RESONANCES; ARRAYS; INDEX AB We present a study of a novel coupling scheme based on the use of two traditional single-gap split ring resonators (SRRs) and two asymmetric double-gap split ring resonators (ASRs) that have different spatial arrangements. Each unit cell consists of two resonator elements. In particular, the two-SRR and two-ASR unit cells are arranged in vertical, horizontal, and diagonal configurations to form a terahertz (THz) macrocell in a large metamaterial (MTM) array. Surprisingly, our results show that the diagonal arrangement in both types of resonators exhibits a strong resonance enhancement, leading to significant improvement in the quality factor (Q-factor) of SRRs and ASRs. Numerical simulations reveal stronger currents being excited for the diagonal macrocell of both types of MTM resonators. This observation is mainly due to optimal coupling between the resonators in the diagonal arrangement that causes subradiant scattering and reduced radiation damping. This coupling scheme could be easily implemented in MTMs across most part of the electromagnetic spectrum in order to minimize undesired radiation losses. We further investigate the effect of mutual interaction on the transmission and the Q-factor of the fundamental resonances in three different kinds of spatial arrangements. C1 [Al-Naib, Ibraheem; Shalaby, Mostafa; Ozaki, Tsuneyuki; Morandotti, Roberto] Inst Natl Rech Sci INRS EMT, Energy Mat & Telecommun Ctr, Varennes, PQ J3X 1S2, Canada. [Singh, Ranjan] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA. RP Al-Naib, I (reprint author), Inst Natl Rech Sci INRS EMT, Energy Mat & Telecommun Ctr, Varennes, PQ J3X 1S2, Canada. EM alnaib@emt.inrs.ca; ranjan@lanl.gov; shalaby@emt.inrs.ca; ozaki@emt.inrs.ca; morandot@emt.inrs.ca RI Singh, Ranjan/B-4091-2010; Al-Naib, Ibraheem/A-2344-2009; OI Singh, Ranjan/0000-0001-8068-7428; Ozaki, Tsuneyuki/0000-0001-8857-3900; Al-Naib, Ibraheem/0000-0002-7499-0655 FU Natural Sciences and Engineering Research Council of Canada; Fonds Quebecois de la Recherche sur la Nature et les Technologies FX This work was supported by the Natural Sciences and Engineering Research Council of Canada and the Fonds Quebecois de la Recherche sur la Nature et les Technologies. NR 43 TC 7 Z9 8 U1 2 U2 33 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 1077-260X J9 IEEE J SEL TOP QUANT JI IEEE J. Sel. Top. Quantum Electron. PD JAN-FEB PY 2013 VL 19 IS 1 AR 8400807 DI 10.1109/JSTQE.2012.2202639 PG 7 WC Engineering, Electrical & Electronic; Optics; Physics, Applied SC Engineering; Optics; Physics GA 128OW UT WOS:000317779700010 ER PT J AU Azad, AK O'Hara, JF Singh, R Chen, HT Taylor, AJ AF Azad, Abul K. O'Hara, John F. Singh, Ranjan Chen, Hou-Tong Taylor, Antoinette J. TI A Review of Terahertz Plasmonics in Subwavelength Holes on Conducting Films SO IEEE JOURNAL OF SELECTED TOPICS IN QUANTUM ELECTRONICS LA English DT Review DE Extraordinary light transmission; plasmonics; surface plasmon polaritons (SPPs); terahertz (THz) ID TIME-DOMAIN SPECTROSCOPY; EXTRAORDINARY OPTICAL-TRANSMISSION; ENHANCED MICROWAVE TRANSMISSION; SURFACE-PLASMON; LIGHT TRANSMISSION; METALLIC GRATINGS; CARRIER DYNAMICS; PERIODIC ARRAY; APERTURES; RADIATION AB In this paper, we present a review of experimental studies of terahertz plasmonic transmission properties through subwavelength holes patterned in conducting films. The frequency-dependent transmission spectrum reveals resonant behavior with an anomalously high peak transmission which is mediated by the excitation of surface plasmon polaritons. We show how terahertz time-domain spectroscopy has been utilized to determine the resonant transmission effects of hole shape, dielectric properties of materials, and thickness of the arrays. Enhanced terahertz transmission was also observed through a single hole, accompanied by annular periodic corrugations. In addition to metals films, we review films comprised of highly doped semiconductors and superconductors. We finally review various modulation schemes to actively control or manipulate the resonant terahertz transmission using external stimuli such as thermal, optical, and electrical fields. This body of work is used to provide perspective on how manipulation of terahertz radiation via surface plasmon polaritons could affect next-generation terahertz photonic devices. C1 [Azad, Abul K.; Singh, Ranjan; Chen, Hou-Tong] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87544 USA. [O'Hara, John F.] Oklahoma State Univ, Dept Elect & Comp Engn, Stillwater, OK 74078 USA. [Taylor, Antoinette J.] Los Alamos Natl Lab, Mat Phys & Applicat Div, Los Alamos, NM 87544 USA. RP Azad, AK (reprint author), Los Alamos Natl Lab, Ctr Integrated Nanotechnol, POB 1663, Los Alamos, NM 87544 USA. EM aazad@lanl.gov; oharaj@okstate.edu; ranjan@lanl.gov; chenht@lanl.gov; ttaylor@lanl.gov RI Chen, Hou-Tong/C-6860-2009; Singh, Ranjan/B-4091-2010; OI Chen, Hou-Tong/0000-0003-2014-7571; Singh, Ranjan/0000-0001-8068-7428; Azad, Abul/0000-0002-7784-7432 FU Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences Nanoscale Science Research Center; Los Alamos and Sandia National Laboratories [DE-AC52-06NA25396]; Los Alamos National Laboratory LDRD Program FX This work was supported in part by the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences Nanoscale Science Research Center operated jointly by Los Alamos and Sandia National Laboratories under Contract DE-AC52-06NA25396 and by Los Alamos National Laboratory LDRD Program. Los Alamos National Laboratory, an affirmative action/equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy. NR 104 TC 10 Z9 10 U1 12 U2 104 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 1077-260X EI 1558-4542 J9 IEEE J SEL TOP QUANT JI IEEE J. Sel. Top. Quantum Electron. PD JAN-FEB PY 2013 VL 19 IS 1 AR 8400416 DI 10.1109/JSTQE.2012.2208181 PG 16 WC Engineering, Electrical & Electronic; Optics; Physics, Applied SC Engineering; Optics; Physics GA 128OW UT WOS:000317779700006 ER PT J AU Zhang, XQ Li, Q Cao, W Gu, JQ Singh, R Tian, Z Han, JG Zhang, WL AF Zhang, Xueqian Li, Quan Cao, Wei Gu, Jianqiang Singh, Ranjan Tian, Zhen Han, Jiaguang Zhang, Weili TI Polarization-Independent Plasmon-Induced Transparency in a Fourfold Symmetric Terahertz Metamaterial SO IEEE JOURNAL OF SELECTED TOPICS IN QUANTUM ELECTRONICS LA English DT Article DE Coupled modes; metamaterials; plasmon-induced transparency (PIT); polarization independent; terahertz (THz) ID RESONANCES AB Metamaterials that reveal fascinating and unique resonant properties allow for adequate control of electromagnetic waves at will. Recently, considerable studies have shown that the plasmon-induced transparency (PIT) effect can be realized by metamaterials via destructive interference between different resonance modes; however, most of them are sensitive to the polarization of incident wave. Here, we demonstrate a polarization-independent PIT metamaterial functioning in the terahertz regime. The proposed structure has a fourfold symmetry and exhibits a typical PIT behavior due to the coupling effect of four different modes, yielding polarization-independent characteristics. C1 [Zhang, Xueqian; Li, Quan; Gu, Jianqiang; Tian, Zhen; Han, Jiaguang; Zhang, Weili] Tianjin Univ, Ctr Terahertz Waves, Tianjin 300072, Peoples R China. [Zhang, Xueqian; Li, Quan; Cao, Wei; Gu, Jianqiang; Tian, Zhen; Han, Jiaguang; Zhang, Weili] Tianjin Univ, Coll Precis Instrument & Optoelect Engn, Tianjin 300072, Peoples R China. [Cao, Wei; Zhang, Weili] Oklahoma State Univ, Sch Elect & Comp Engn, Stillwater, OK 74078 USA. [Singh, Ranjan] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. [Singh, Ranjan] Mat Phys & Applicat Div, Los Alamos, NM 87545 USA. RP Zhang, XQ (reprint author), Tianjin Univ, Ctr Terahertz Waves, Tianjin 300072, Peoples R China. EM alearn1988@126.com; thztju@tju.edu.cn; wei.cao@okstate.edu; gjq@tju.edu.cn; ranjan.ranjansingh@gmail.com; zhen_tian@yahoo.com.cn; jiaghan@tju.edu.cn; weili.zhang@okstate.edu RI Singh, Ranjan/B-4091-2010; Zhang, Weili/C-5416-2011; Tian, Zhen/D-8707-2015 OI Singh, Ranjan/0000-0001-8068-7428; Zhang, Weili/0000-0002-8591-0200; Tian, Zhen/0000-0002-2861-4325 FU National Science Foundation of China [61138001, 61107053, 61028011, 61107085, 61007034]; U.S. National Science Foundation FX This work was supported in part by the National Science Foundation of China under Grant 61138001, Grant 61107053, Grant 61028011, Grant 61107085, and Grant 61007034, and in part by the U.S. National Science Foundation. NR 30 TC 12 Z9 14 U1 0 U2 38 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 1077-260X J9 IEEE J SEL TOP QUANT JI IEEE J. Sel. Top. Quantum Electron. PD JAN-FEB PY 2013 VL 19 IS 1 AR 8400707 DI 10.1109/JSTQE.2012.2200656 PG 7 WC Engineering, Electrical & Electronic; Optics; Physics, Applied SC Engineering; Optics; Physics GA 128OW UT WOS:000317779700009 ER PT J AU Eppich, GR Williams, RW Gaffney, AM Schorzman, KC AF Eppich, Gary R. Williams, Ross W. Gaffney, Amy M. Schorzman, Kerri C. TI U-235-Pa-231 age dating of uranium materials for nuclear forensic investigations SO JOURNAL OF ANALYTICAL ATOMIC SPECTROMETRY LA English DT Article ID PLASMA-MASS SPECTROMETRY; FEMTOGRAM QUANTITIES; ANION-EXCHANGE; HCL-HF; PROTOACTINIUM; SEPARATION; SAMPLES AB Age dating of nuclear material can provide insight into source and suspected use in nuclear forensic investigations. We report here a method for the determination of the date of most recent chemical purification for uranium materials using the U-235-Pa-231 chronometer. Protactinium is separated from uranium and neptunium matrices using anion exchange resin, followed by sorption of Pa to an SiO2 medium. The concentration of Pa-231 is measured by isotope dilution mass spectrometry using Pa-233 spikes prepared from an aliquot of Np-237 and calibrated in-house using the rock standard Table Mountain Latite and the uranium isotopic standard U100. Combined uncertainties of age dates using this method are 1.5 to 3.5 %, an improvement over alpha spectrometry measurement methods. Model ages of five uranium standard reference materials are presented; all standards have concordant U-235-Pa-231 and U-234-Th-230 model ages. C1 [Eppich, Gary R.; Williams, Ross W.; Gaffney, Amy M.; Schorzman, Kerri C.] Lawrence Livermore Natl Lab, Div Chem Sci, Livermore, CA USA. RP Eppich, GR (reprint author), Lawrence Livermore Natl Lab, Div Chem Sci, 7000 East Ave, Livermore, CA USA. EM eppich1@llnl.gov RI Gaffney, Amy/F-8423-2014; OI Gaffney, Amy/0000-0001-5714-0029; Eppich, Gary/0000-0003-2176-6673 FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344. LLNL-JRNL-615952] FX The authors would like to thank two anonymous reviewers who provided useful comments leading to an improved manuscript. Major support for this work was provided by the Office of Nonproliferation and International Security (NA-24), National Nuclear Security Administration, and the U.S. Department of Energy. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. LLNL-JRNL-615952. NR 12 TC 17 Z9 17 U1 8 U2 49 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 0267-9477 J9 J ANAL ATOM SPECTROM JI J. Anal. At. Spectrom. PY 2013 VL 28 IS 5 BP 666 EP 674 DI 10.1039/c3ja50041a PG 9 WC Chemistry, Analytical; Spectroscopy SC Chemistry; Spectroscopy GA 127CV UT WOS:000317674200006 ER PT J AU Lu, Y Zorba, V Mao, XL Zheng, RE Russo, RE AF Lu, Yuan Zorba, Vassilia Mao, Xianglei Zheng, Ronger Russo, Richard E. TI UV fs-ns double-pulse laser induced breakdown spectroscopy for high spatial resolution chemical analysis SO JOURNAL OF ANALYTICAL ATOMIC SPECTROMETRY LA English DT Article ID ORTHOGONAL BEAM GEOMETRY; COPPER-BASED-ALLOYS; SPECTROCHEMICAL ANALYSIS; TEMPORAL DEPENDENCE; PLASMA; FEMTOSECOND; LIBS; ABLATION; EMISSION; TIME AB We study the use of an ultraviolet (UV) femtosecond (fs)-nanosecond (ns) double-pulse scheme to improve the analytical capabilities of Laser Induced Breakdown Spectroscopy (LIBS) in the few-micron (<2 mu m) spatial resolution regime. We show that a double-pulse orthogonal configuration can enhance the spectral emission intensity by roughly 360 times as compared to a single-fs laser pulse LIBS of silicon (Si). Although the spectral emission lifetime in single-pulse LIBS is less than 20 ns, the second pulse provides signal enhancement hundreds of nanoseconds later, indicating that a significant number of non-radiative species (neutrals and/or particles) exist in these small length-scale plasmas long after the fslaser pulse is over. The double-pulse configuration is a practical way to improve the limits of detection of LIBS for micron/submicron spatial resolution. C1 [Lu, Yuan; Zorba, Vassilia; Mao, Xianglei; Russo, Richard E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Lu, Yuan; Zheng, Ronger] Ocean Univ China, Qingdao 266100, Shandong, Peoples R China. RP Russo, RE (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM RERusso@lbl.gov RI Zorba, Vassilia/C-4589-2015 FU Chemical Science Division, Office of Basic Energy Sciences, Office of Nuclear Nonproliferation, and the U.S. Department of Energy [DE-AC02-05CH11231]; Laboratory Directed Research and Development (LDRD); Berkeley Lab, Office of Science, of the U.S. Department of Energy; China Scholarship Council (CSC) FX This research has been supported by the Chemical Science Division, Office of Basic Energy Sciences, Office of Nuclear Nonproliferation, and the U.S. Department of Energy under Contract no. DE-AC02-05CH11231. This work was also supported by Laboratory Directed Research and Development (LDRD) funding from Berkeley Lab, provided by the Director, Office of Science, of the U.S. Department of Energy. The work of Y. Lu was supported by the China Scholarship Council (CSC). NR 51 TC 31 Z9 32 U1 3 U2 49 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 0267-9477 J9 J ANAL ATOM SPECTROM JI J. Anal. At. Spectrom. PY 2013 VL 28 IS 5 BP 743 EP 748 DI 10.1039/c3ja30315b PG 6 WC Chemistry, Analytical; Spectroscopy SC Chemistry; Spectroscopy GA 127CV UT WOS:000317674200016 ER PT J AU Wang, CP Zaharia, SG Lyons, LR Angelopoulos, V AF Wang, Chih-Ping Zaharia, Sorin G. Lyons, Larry R. Angelopoulos, Vassilis TI Spatial distributions of ion pitch angle anisotropy in the near-Earth magnetosphere and tail plasma sheet SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article ID DAWN-DUSK ASYMMETRY; FIELD; MODEL; MAGNETOTAIL; PRECIPITATION; SCATTERING; PARTICLES; ISEE-1; MOTION; STORM AB We have quantified anisotropy of ion pitch angle distributions observed by the Time History of Events and Macroscale Interactions during Substorms (THEMIS) spacecraft and determined statistically how anisotropy varies with particle energy, as well as spatial distributions and dependences on geomagnetic activity. In the tail plasma sheet, ions from a few keV to a few tens of keV are mostly isotropic. The locations and energy ranges for these isotropic ions and their changes with Dst are consistent with ions being isotropized by current sheet scattering predicted using empirical magnetic field models. Ions of a few hundreds of keV in the tail have cigar-shaped or unidirectional pitch angle distribution (PAD) and are likely a result of Speiser motion. The majority of ions in the near-Earth magnetosphere are expected to conserve their first and second adiabatic invariants as they move with pitch angle dependent drift. This gives drift shell splitting, which plays an important role in generating pancake-shaped PAD observed from similar to 1 keV up to hundreds of keV. The magnetic local time of the pancake PAD rotates with increasing energy. Loss of near 90 degrees ions due to magnetopause shadowing can further explain the butterfly-shaped PAD observed at the postmidnight sector at energies above 30 keV. For ions below a few hundreds of eV in the tail plasma sheet and the near-Earth magnetosphere, their PAD is dominantly bidirectional, which is likely due to ionosphere outflow. High-energy ions on the dayside become less anisotropic during higher AE, when pitch angle scattering by electromagnetic ion cyclotron waves may play an important role. Citation: Wang, C.-P., S. G. Zaharia, L. R. Lyons, and V. Angelopoulos (2012), Spatial distributions of ion pitch angle anisotropy in the near-Earth magnetosphere and tail plasma sheet, J. Geophys. Res. Space Physics, 118, 244-255, doi:10.1029/2012JA018275. C1 [Wang, Chih-Ping; Lyons, Larry R.] Univ Calif Los Angeles, Dept Atmospher & Ocean Sci, Los Angeles, CA 90024 USA. [Zaharia, Sorin G.] Los Alamos Natl Lab, Space Sci & Applicat ISR 1, Los Alamos, NM USA. [Angelopoulos, Vassilis] Univ Calif Los Angeles, Dept Earth & Space Sci, Los Angeles, CA 90024 USA. RP Wang, CP (reprint author), Univ Calif Los Angeles, Dept Atmospher & Ocean Sci, Los Angeles, CA 90024 USA. EM cat@atmos.ucla.edu FU NASA [NNX07AF66G, NNX07AG42G, NNX09AQ41H, NNX08A135G, NNH09AL06I, NAS5-02099]; NSF [ATM-0819864, ATM-1003595, ATM-0902941, AGS-1131873]; DLR [50 OC 0302]; ISSI FX The work by C.-P. Wang and L. R. Lyons have been supported by NASA grants NNX07AF66G, NNX07AG42G, NNX09AQ41H, and NNX08A135G, and NSF grants ATM-0819864 and ATM-1003595. The work by S. G. Zaharia has been supported by NASA grant NNH09AL06I and NSF grants ATM-0902941 and AGS-1131873. We acknowledge NASA contract NAS5-02099 for THEMIS, and C. W. Carlson and J. P. McFadden for the use of ESA data, D. Larson and R. P. Lin for use of the SST data, K. H. Glassmeier, U. Auster and W. Baumjohann for the use of FGM data provided under DLR contract 50 OC 0302. OMNI data. We thank Drew Turner for useful discussion in processing the SST data. AE index was provided by World Data Center for Geomagnetism, Kyoto. We thank the support of ISSI International Teams Program: Plasma Entry and Transport in the Plasma Sheet. NR 43 TC 19 Z9 19 U1 1 U2 7 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD JAN PY 2013 VL 118 IS 1 BP 244 EP 255 DI 10.1029/2012JA018275 PG 12 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 129RC UT WOS:000317858600024 ER PT J AU Hercik, D Travnicek, PM Johnson, JR Kim, EH Hellinger, P AF Hercik, David Travnicek, Pavel M. Johnson, Jay R. Kim, Eun-Hwa Hellinger, Petr TI Mirror mode structures in the asymmetric Hermean magnetosheath: Hybrid simulations SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article ID PERPENDICULAR BOW SHOCK; MESSENGERS 1ST FLYBY; LOW-FREQUENCY WAVES; SOLAR-WIND; MAGNETIC-FIELD; ANISOTROPY INSTABILITIES; LINEAR INSTABILITY; MACH NUMBER; MAGNETOSPHERE; MAGNETOPAUSE AB Results of two global three-dimensional hybrid simulations of the solar wind interaction with the Hermean magnetosphere are presented for southward and northward interplanetary magnetic field (IMF) orientations. Important dawn-dusk asymmetries of the Hermean bow shock and magnetosheath are observed depending on the IMF orientation. For the southward IMF, the dawnside has a thicker magnetosheath with higher beta values and slower bulk velocities compared to the duskside, whereas for the northward IMF, the duskside has a thicker and higher beta magnetosheath with slower bulk velocities. Mirror mode activity consequently appears at the dawnside for the southward IMF and at the duskside for the northward IMF. A mechanism for the bow shock and magnetosheath asymmetries is proposed and discussed in the context of the Hermean and terrestrial magnetosheaths. Citation: Hercik, D., P. M. Travnicek, J. R. Johnson, E.-H. Kim, and P. Hellinger (2013), Mirror mode structures in the asymmetric Hermean magnetosheath: Hybrid simulations, J. Geophys. Res. Space Physics, 118, 405-417, doi:10.1029/2012JA018083. C1 [Hercik, David; Travnicek, Pavel M.; Hellinger, Petr] Acad Sci Czech Republic, Inst Astron, CR-12023 Prague, Czech Republic. [Hercik, David; Travnicek, Pavel M.; Hellinger, Petr] Acad Sci Czech Republic, Inst Atmospher Phys, Prague, Czech Republic. [Hercik, David] Czech Tech Univ, Fac Nucl Sci & Phys Engn, CR-11519 Prague, Czech Republic. [Travnicek, Pavel M.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Johnson, Jay R.; Kim, Eun-Hwa] Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. RP Hercik, D (reprint author), Acad Sci Czech Republic, Inst Astron, Budecska 6, CR-12023 Prague, Czech Republic. EM hercik@asu.cas.cz RI Hellinger, Petr/F-5267-2014; Hercik, David/G-1224-2014; Travnicek, Pavel/G-8608-2014 OI Hellinger, Petr/0000-0002-5608-0834; FU European Commission's Seventh Framework Programme (FP7) under the grant agreement SWIFF [263340]; European Commission's Seventh Framework Programme (FP7) under the grant agreement SHOCK [284515]; Czech Ministry of Education, Youth and Sports [ME09009, RVO: 67985815]; NASA [NNX11A1164G, NNH06ZDA001N, NNX12AD08G, NNH09AM53I, NNH09AK63I, NNH11AQ46I]; NSF [ATM0902730]; DOE [DE-AC02-09CH11466]; [RVO: 68378289] FX The research at the Astronomical Institute, ASCR leading to these results has received funding from the European Commission's Seventh Framework Programme (FP7) under the grant agreement SWIFF (project 263340) and SHOCK (project 284515) and from Czech Ministry of Education, Youth and Sports under project ME09009 and project RVO: 67985815. At Institute of Atmospheric Physics, work was supported by RVO: 68378289. The work at the University California Berkeley was supported by NASA grants NNX11A1164G, NNH06ZDA001N, and NNX12AD08G. The work at the Princeton University was supported by NASA grants (NNH09AM53I, NNH09AK63I, and NNH11AQ46I), NSF grant ATM0902730, and DOE contract DE-AC02-09CH11466. NR 59 TC 4 Z9 4 U1 2 U2 7 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD JAN PY 2013 VL 118 IS 1 BP 405 EP 417 DI 10.1029/2012JA018083 PG 13 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 129RC UT WOS:000317858600038 ER PT J AU Martha, SK Nanda, J Kim, Y Unocic, RR Pannala, S Dudney, NJ AF Martha, Surendra K. Nanda, Jagjit Kim, Yoongu Unocic, Raymond R. Pannala, Sreekanth Dudney, Nancy J. TI Solid electrolyte coated high voltage layered-layered lithium-rich composite cathode: Li1.2Mn0.525Ni0.175Co0.1O2 SO JOURNAL OF MATERIALS CHEMISTRY A LA English DT Article ID LI-ION BATTERIES; HIGH-CAPACITY; RATE CAPABILITY; CO ELECTRODES; SURFACE; MN; SPINEL; CELL; NI; PERFORMANCE AB The electrochemical rate performance and capacity retention of the "layered-layered" lithium rich Li1.2Mn0.525Ni0.175Co0.1O2 (Li-rich NMC) material are significantly improved by a nanometer layer coating of a lithium conducting solid electrolyte, lithium phosphorus oxynitride (LiPON). The LiPON layer is deposited on the Li-rich NMC particles by the RF-magnetron sputtering method. The presence of the LiPON layer provides interfacial stability under high current (rate) and voltage cycling conditions and thereby improves the capacity retention over cycle life compared to pristine or uncoated Li-rich NMC. Specifically, the LiPON coated Li-rich NMC composite electrode showed stable reversible capacities of >275 mAh g(-1) when cycled to 4.9 V for more than 300 cycles, and showed at least threefold improvements in the rate performance compared to the uncoated electrode compositions. Increasing the LiPON layer thickness beyond a few nanometers leads to capacity fade due to increasing electronic resistance. Detailed microstructural and electrochemical impedance spectroscopy studies are undertaken to characterize and understand the role of LiPON in improving the interfacial stability and electrochemical activity at the interface. C1 [Martha, Surendra K.; Nanda, Jagjit; Kim, Yoongu; Unocic, Raymond R.; Dudney, Nancy J.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Pannala, Sreekanth] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. RP Martha, SK (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. EM nandaj@ornl.gov RI Pannala, Sreekanth/F-9507-2010; Dudney, Nancy/I-6361-2016 OI Dudney, Nancy/0000-0001-7729-6178 FU U.S. Department of Energy [DE-AC05-00OR22725]; Vehicle Technologies Program for the Office of Energy Efficiency and Renewable Energy; ORNL's Shared Research Equipment (ShaRE) User Program; Office of Basic Energy Sciences, the U.S. Department of Energy FX This research at Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy under contract DE-AC05-00OR22725, was sponsored by the Vehicle Technologies Program for the Office of Energy Efficiency and Renewable Energy. The electron microscopy work was supported by ORNL's Shared Research Equipment (ShaRE) User Program, which was sponsored by the Office of Basic Energy Sciences, the U.S. Department of Energy. Materials used in this study were supplied courtesy of Toda Kyogo Corporation, Japan. The authors also acknowledge the assistance of G. M. Veith and Loic Baggetto (MSTD, ORNL) for discussions on XPS analysis. The authors also would like to acknowledge Dorothy Coffey for FIB and TEM specimen preparation. NR 37 TC 47 Z9 47 U1 15 U2 186 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2050-7488 EI 2050-7496 J9 J MATER CHEM A JI J. Mater. Chem. A PY 2013 VL 1 IS 18 BP 5587 EP 5595 DI 10.1039/c3ta10586e PG 9 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Energy & Fuels; Materials Science GA 126AY UT WOS:000317584700018 ER PT J AU Karwacki, CJ Ganesh, P Kent, PRC Gordon, WO Peterson, GW Niu, JJ Gogotsi, Y AF Karwacki, Christopher J. Ganesh, P. Kent, Paul R. C. Gordon, Wesley O. Peterson, Gregory W. Niu, Jun Jie Gogotsi, Yury TI Structure-activity relationship of Au/ZrO2 catalyst on formation of hydroxyl groups and its influence on CO oxidation SO JOURNAL OF MATERIALS CHEMISTRY A LA English DT Article ID SUPPORTED GOLD NANOPARTICLES; AUGMENTED-WAVE METHOD; GAS SHIFT REACTION; ZIRCONIA POLYMORPHS; SURFACE-CHEMISTRY; TETRAGONAL ZRO2; AU; ADSORPTION; WATER; CLUSTERS AB The effect of changes in morphology and surface hydroxyl species upon thermal treatment of zirconia on the oxidation activity of Au/ZrO2 catalyst was studied. We observed using transmission Fourier transform infrared (FTIR) spectroscopy progressive changes in the presence of monodentate (type I), bidentate (type II) and hydrogen bridged species (type III) for each of the thermally treated (85 to 500 degrees C) supports consisting of bare zirconia and Au/ZrO2 catalysts. Furthermore, structural changes in zirconia were accompanied by an increase in crystal size (7 to 58 nm) and contraction of the supports porosity (SSA 532 to 7 m(2) g(-1)) with increasing thermal treatment. Deposition of gold nanoparticles under similar preparation conditions on different thermally treated zirconia resulted in changes in the mean gold cluster size, ranging from 3.7 to 5.6 nm. Changes in the surface hydroxyl species, support structure and size of the gold centers are important parameters responsible for the observed decrease (>90%) in CO conversion activity for the Au/ZrO2 catalysts. Density functional theory calculations provide evidence of increased CO binding to Au nanoclusters in the presence of surface hydroxyls on zirconia, which increases charge transfer at the perimeter of the gold nanocluster on zirconia support. This further helps in reducing a model CO-oxidation reaction barrier in the presence of surface hydroxyls. This work demonstrates the need to understand the structure-activity relationship of both the support and active particles for the design of catalytic materials. C1 [Karwacki, Christopher J.; Gordon, Wesley O.; Peterson, Gregory W.] Edgewood Chem Biol Ctr, Aberdeen Proving Ground, MD 21010 USA. [Ganesh, P.; Kent, Paul R. C.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Kent, Paul R. C.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. [Niu, Jun Jie; Gogotsi, Yury] Drexel Univ, Dept Mat Sci & Engn, AJ Drexel Nanotechnol Inst, Philadelphia, PA 19104 USA. RP Karwacki, CJ (reprint author), Edgewood Chem Biol Ctr, 5183 Blackhawk Rd, Aberdeen Proving Ground, MD 21010 USA. EM christopher.j.karwacki.civ@mail.mil RI Kent, Paul/A-6756-2008; Ganesh, Panchapakesan/L-5571-2013; Gogotsi, Yury/B-2167-2008; Ganesh, Panchapakesan/E-3435-2012; OI Kent, Paul/0000-0001-5539-4017; Gogotsi, Yury/0000-0001-9423-4032; Ganesh, Panchapakesan/0000-0002-7170-2902; Peterson, Gregory/0000-0003-3467-5295 FU US Army Research Development Engineering Command; Aberdeen Proving Ground, MD; Army Research Office; Research Triangle Park, NC; Joint Science and Technology Office; Fluid Interface Reactions, Structures and Transport (FIRST) Center, an Energy Frontier Research Center; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the US Army Research Development Engineering Command, Aberdeen Proving Ground, MD, the Army Research Office, Research Triangle Park, NC and the Joint Science and Technology Office. PG and PRCK (DFT calculations) were supported as part of the Fluid Interface Reactions, Structures and Transport (FIRST) Center, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. Computations used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract no. DE-AC02-05CH11231. NR 48 TC 13 Z9 13 U1 5 U2 64 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2050-7488 J9 J MATER CHEM A JI J. Mater. Chem. A PY 2013 VL 1 IS 19 BP 6051 EP 6062 DI 10.1039/c3ta00081h PG 12 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Energy & Fuels; Materials Science GA 130RF UT WOS:000317936000034 ER PT J AU Byun, TS Toloczko, MB Saleh, TA Maloy, SA AF Byun, Thak Sang Toloczko, Mychailo B. Saleh, Tarik A. Maloy, Stuart A. TI Irradiation dose and temperature dependence of fracture toughness in high dose HT9 steel from the fuel duct of FFTF SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID CORE MATERIALS; SPECIMEN; REACTORS AB To expand the knowledge base for fast reactor core materials, fracture toughness has been evaluated for high dose HT9 steel using miniature disk compact tension (DCT) specimens. The HT9 steel DCT specimens were machined from the ACO-3 fuel duct of the Fast Flux Test Facility (FFTF), which achieved high doses in the range of 3-148 dpa at 378-504 degrees C. The static fracture resistance (J-R) tests have been performed in a servohydraulic testing machine in vacuum at selected temperatures including room temperature, 200 degrees C, and each irradiation temperature. Brittle fracture with a low toughness less than 50 MPa root m occurred in room temperature tests when irradiation temperature was below 400 degrees C, while ductile fracture with stable crack growth was observed when irradiation temperature was higher. No fracture toughness less than 100 MPa root m was measured when the irradiation temperature was above 430 degrees C. It was shown that the influence of irradiation temperature was dominant in fracture toughness while the irradiation dose has only limited influence over the wide dose range 3-148 dpa. A slow decrease of fracture toughness with test temperature above room temperature was observed for the nonirradiated and high temperature (>430 degrees C) irradiation cases, which indicates that the ductile-brittle transition temperatures (DBTTs) in those conditions are lower than room temperature. A comparison with the collection of existing data confirmed the dominance of irradiation temperature in the fracture toughness of HT9 steels. Published by Elsevier B.V. C1 [Byun, Thak Sang] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Toloczko, Mychailo B.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Saleh, Tarik A.; Maloy, Stuart A.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Byun, TS (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. EM byunts@ornl.gov RI Maloy, Stuart/A-8672-2009; OI Maloy, Stuart/0000-0001-8037-1319; Saleh, Tarik/0000-0003-2108-4293 FU US Department of Energy, Office of Nuclear Energy [DE-AC05-00OR22725]; UT-Battelle, LLC FX This research was sponsored by US Department of Energy, Office of Nuclear Energy under Contract DE-AC05-00OR22725 with UT-Battelle, LLC. The authors would like to express special thanks to Dr. L. Tan of ORNL for his technical review and thoughtful comments. NR 24 TC 6 Z9 6 U1 5 U2 19 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 J9 J NUCL MATER JI J. Nucl. Mater. PD JAN PY 2013 VL 432 IS 1-3 BP 1 EP 8 DI 10.1016/j.jnucmat.2012.07.019 PG 8 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA 128XB UT WOS:000317801900001 ER PT J AU Chen, X Sokolov, MA Sham, S Erdman, DL Busby, JT Mo, K Stubbins, JF AF Chen, Xiang Sokolov, Mikhail A. Sham, Sam Erdman, Donald L., III Busby, Jeremy T. Mo, Kun Stubbins, James F. TI Experimental and modeling results of creep-fatigue life of Inconel 617 and Haynes 230 at 850 degrees C SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID NICKEL-BASE SUPERALLOY; LOW-CYCLE FATIGUE; STRUCTURAL-MATERIALS; HIGH-TEMPERATURE; BEHAVIOR; DEFORMATION; REACTORS; ALLOYS; TIME AB Creep-fatigue testing of Ni-based superalloy Inconel 617 and Haynes 230 were conducted in the air at 850 degrees C. Tests were performed with fully reversed axial strain control at a total strain range of 0.5%, 1.0% or 1.5% and hold time at maximum tensile strain for 3, 10 or 30 min. In addition, two creep-fatigue life prediction methods, i.e. linear damage summation and frequency-modified tensile hysteresis energy modeling, were evaluated and compared with experimental results. Under all creep-fatigue tests, Haynes 230 performed better than Inconel 617. Compared to the low cycle fatigue life, the cycles to failure for both materials decreased under creep-fatigue test conditions. Longer hold time at maximum tensile strain would cause a further reduction in both material creep-fatigue life. The linear damage summation could predict the creep-fatigue life of Inconel 617 for limited test conditions, but considerably underestimated the creep-fatigue life of Haynes 230. In contrast, frequency-modified tensile hysteresis energy modeling showed promising creep-fatigue life prediction results for both materials. Published by Elsevier B.V. C1 [Chen, Xiang; Mo, Kun; Stubbins, James F.] Univ Illinois, Dept Nucl Plasma & Radiol Engn, Urbana, IL 61801 USA. [Chen, Xiang; Sokolov, Mikhail A.; Sham, Sam; Erdman, Donald L., III; Busby, Jeremy T.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Chen, X (reprint author), 1 Bethel Valley Rd,POB 2008,Bldg 4500S,MS 6151, Oak Ridge, TN 37831 USA. EM chenx@ornl.gov RI Mo, Kun/A-9737-2011; Chen, Xiang/D-4531-2013; OI Mo, Kun/0000-0003-0412-8987; Chen, Xiang/0000-0002-8662-5209 FU U.S. Department of Energy [DE-FC07-07ID14819, NEUP 09-516] FX The work was supported by the U.S. Department of Energy grants DE-FC07-07ID14819 and NEUP 09-516. The microanalysis was carried out in the Shared Research Equipment User Facility at Oak Ridge National Laboratory which is supported by the Scientific User Facilities Division of the Office of Science, U.S. Department of Energy. The authors are thankful for Dr. Richard Wright and Dr. Laura Carroll from Idaho National Laboratory and Dr. Henry White from Haynes International Inc. for providing test materials. The authors also would like to thank Christopher Stevens and Eric Manneschmidt from Oak Ridge National Laboratory for their technical support. NR 33 TC 16 Z9 16 U1 3 U2 38 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 J9 J NUCL MATER JI J. Nucl. Mater. PD JAN PY 2013 VL 432 IS 1-3 BP 94 EP 101 DI 10.1016/j.jnucmat.2012.08.040 PG 8 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA 128XB UT WOS:000317801900016 ER PT J AU Kirchhofer, R Hunn, JD Demkowicz, PA Cole, JI Gorman, BP AF Kirchhofer, Rita Hunn, John D. Demkowicz, Paul A. Cole, James I. Gorman, Brian P. TI Microstructure of TRISO coated particles from the AGR-1 experiment: SiC grain size and grain boundary character SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID FUEL-PARTICLES; SILICON-CARBIDE; PERFORMANCE; DIFFUSION; SILVER; EBSD AB Pre-irradiation SiC microstructures in tristructural-isotropic (TRISO) coated fuel particles from the Advanced Gas Reactor Fuel Development and Qualification program's first irradiation experiment (AGR-1) were quantitatively characterized using electron backscatter diffraction (EBSD) and transmission electron microscopy (TEM). From EBSD, it was determined that only the cubic polymorph of as-deposited SiC was present and the SiC had a high fraction of coincident site lattice (CSL) Sigma 3 grain boundaries. Additionally, the local area misorientation (LAM), which is a qualitative measurement of strain in the SiC lattice, was mapped for each sample fuel variant. The morphology of the SiC/IPyC interfaces were characterized by TEM following site-specific focused ion beam (FIB) specimen preparation. It was determined that the SiC layer had a heavily faulted microstructure typical of chemical vapor deposition (CVD) SiC and that the average grain diameter increased radially from the SiC/IPyC interface for the samples manufactured with similar CVD conditions, while the last sample showed a nearly constant grain size across the layer. (c) 2012 Elsevier B.V. All rights reserved. C1 [Kirchhofer, Rita; Gorman, Brian P.] Colorado Sch Mines, Golden, CO 80401 USA. [Hunn, John D.] Oak Ridge Natl Lab, Fuel Cycle & Isotopes Div, Oak Ridge, TN USA. [Demkowicz, Paul A.] Idaho Natl Lab, Nucl Fuels & Mat Div, Idaho Falls, ID 83415 USA. [Cole, James I.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. RP Kirchhofer, R (reprint author), Colorado Sch Mines, 1500 Illinois St, Golden, CO 80401 USA. EM rkirchho@mines.edu OI Cole, James/0000-0003-1178-5846 FU US Department of Energy through Nuclear Energy University Program (NEUP); Idaho National Laboratory (INL); US Department of Energy Advanced Gas Reactor Fuel Development and Qualification Program FX This work was funded by the US Department of Energy through Nuclear Energy University Program (NEUP) and Idaho National Laboratory (INL). Sample analysis was performed at Idaho National Laboratory and Colorado School of Mines. Special thanks to M. K. Meyer (INL). Coated particle fabrication at Oak Ridge National Laboratory (ORNL) was supported by the US Department of Energy Advanced Gas Reactor Fuel Development and Qualification Program. NR 27 TC 21 Z9 22 U1 2 U2 28 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 J9 J NUCL MATER JI J. Nucl. Mater. PD JAN PY 2013 VL 432 IS 1-3 BP 127 EP 134 DI 10.1016/j.jnucmat.2012.08.052 PG 8 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA 128XB UT WOS:000317801900020 ER PT J AU Wei, CC Aitkaliyeva, A Luo, ZP Ewh, A Sohn, YH Kennedy, JR Sencer, BH Myers, MT Martin, M Wallace, J General, MJ Shao, L AF Wei, Chao-Chen Aitkaliyeva, Assel Luo, Zhiping Ewh, Ashley Sohn, Y. H. Kennedy, J. R. Sencer, Bulent H. Myers, M. T. Martin, M. Wallace, J. General, M. J. Shao, Lin TI Understanding the phase equilibrium and irradiation effects in Fe-Zr diffusion couples SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article AB We have studied the radiation effects in Fe-Zr diffusion couples, formed by thermal annealing of a mechanically bonded binary system at 850 degrees C for 15 days. After irradiation with 3.5 MeV Fe ions at 600 degrees C, a cross sectional specimen was prepared by using a focused-ion-beam-based lift out technique and was characterized using scanning/transmission electron microscopy, selected-area diffraction and X-ray energy dispersive spectroscopy analyses. Comparison studies were performed in localized regions within and beyond the ion projected range and the following observations were obtained: (1) the interaction layer consists of FeZr3, FeZr2, Fe2Zr, and Fe23Zr6; (2) large Fe23Zr6 particles with smaller core particles of Zr-rich Fe2Zr are found within the alpha-Fe matrix; (3) Zr diffusion is significantly enhanced in the ion bombarded region, leading to the formation of an Fe-Zr compound; (4) grains located within the interaction layer are much smaller in the ion bombarded region and are associated with new crystal growth and nanocrystal formation; and (5) large alpha-Fe particles form on the surface of the Fe side, but the particles are limited to the region close to the interaction layer. These studies reveal the complexity of the interaction phase formation in an Fe-Zr binary system and the accelerated microstructural changes under irradiation. (c) 2012 Elsevier B.V. All rights reserved. C1 [Wei, Chao-Chen; Aitkaliyeva, Assel; Luo, Zhiping; General, M. J.; Shao, Lin] Texas A&M Univ, Mat Sci & Engn Program, College Stn, TX 77843 USA. [Luo, Zhiping] Texas A&M Univ, Microscopy & Imaging Ctr, College Stn, TX 77843 USA. [Ewh, Ashley; Sohn, Y. H.] Univ Cent Florida, Dept Mat Sci & Engn, Orlando, FL 32816 USA. [Aitkaliyeva, Assel; Kennedy, J. R.; Sencer, Bulent H.] Idaho Natl Lab, Fundamental Fuel Properties Dept, Nucl Fuel & Mat Div, Idaho Falls, ID 83415 USA. [Myers, M. T.; Martin, M.; Wallace, J.; Shao, Lin] Texas A&M Univ, Dept Nucl Engn, College Stn, TX 77843 USA. RP Shao, L (reprint author), Texas A&M Univ, Dept Nucl Engn, College Stn, TX 77843 USA. EM lshao@tamu.edu RI Sohn, Yongho/A-8517-2010; Luo, Zhiping/C-4435-2014; Paz y Puente, Ashley/M-2022-2015; OI Sohn, Yongho/0000-0003-3723-4743; Luo, Zhiping/0000-0002-8264-6424; Paz y Puente, Ashley/0000-0001-7108-7164; Aitkaliyeva, Assel/0000-0003-1481-6804 FU US Department of Energy under DOE-NE Idaho Operations Office [AC07-05ID14517] FX This work was supported by the US Department of Energy under DOE-NE Idaho Operations Office Contract DE-AC07-05ID14517. NR 12 TC 5 Z9 5 U1 1 U2 18 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 J9 J NUCL MATER JI J. Nucl. Mater. PD JAN PY 2013 VL 432 IS 1-3 BP 205 EP 211 DI 10.1016/j.jnucmat.2012.07.027 PG 7 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA 128XB UT WOS:000317801900030 ER PT J AU Baker, MP King, JC Gorman, BP Marshall, DW AF Baker, M. P. King, J. C. Gorman, B. P. Marshall, D. W. TI Selection and properties of alternative forming fluids for TRISO fuel kernel production SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID GEL MICROSPHERE PELLETIZATION; INTERNAL GELATION; ZIRCONIA MICROSPHERES; URANIUM-DIOXIDE; FABRICATION; CERIA; PELLETS; YTTRIA AB Current Very High Temperature Reactor (VHTR) designs incorporate TRi-structural ISOtropic (TRISO) fuel, which consists of a spherical fissile fuel kernel surrounded by layers of pyrolytic carbon and silicon carbide. An internal sol-gel process forms the fuel kernel using wet chemistry to produce uranium oxyhydroxide gel spheres by dropping a cold precursor solution into a hot column of trichloroethylene (TCE). Over time, gelation byproducts inhibit complete gelation, and the TCE must be purified or discarded. The resulting TCE waste stream contains both radioactive and hazardous materials and is thus considered a mixed hazardous waste. Changing the forming fluid to a non-hazardous alternative could greatly improve the economics of TRISO fuel kernel production. Selection criteria for a replacement forming fluid narrowed a list of similar to 10,800 chemicals to yield ten potential replacement forming fluids: 1-bromododecane, 1-bromotetradecane, 1-bromoundecane, 1-chlorooctadecane, 1-chlorotetradecane, 1-iododecane, 1-iodododecane, 1-iodohexadecane, 1-iodooctadecane, and squalane. The density, viscosity, and surface tension for each potential replacement forming fluid were measured as a function of temperature between 25 degrees C and 80 degrees C. Calculated settling velocities and heat transfer rates give an overall column height approximation. 1-bromotetradecane, 1-chlorooctadecane, and 1-iodododecane show the greatest promise as replacements, and future tests will verify their ability to form satisfactory fuel kernels. (C) 2012 Elsevier B.V. All rights reserved. C1 [Baker, M. P.; King, J. C.; Gorman, B. P.] Colorado Sch Mines, Golden, CO 80401 USA. [Marshall, D. W.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. RP King, JC (reprint author), Colorado Sch Mines, 1500 Illinois St, Golden, CO 80401 USA. EM kingjc@mines.edu FU Colorado School of Mines' Nuclear Science and Engineering Fellowship; U.S. Nuclear Regulatory Commission (NRC) FX Michael Baker's research is supported by a Colorado School of Mines' Nuclear Science and Engineering Fellowship, which is co-sponsored by the U.S. Nuclear Regulatory Commission (NRC). Additional acknowledgement is given to Dr. Jeffrey Phillips at Idaho National Laboratory, and Clay Richardson and Scott Niedzialek at Babcock & Wilcox, for their input and advice. NR 45 TC 1 Z9 1 U1 1 U2 10 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 J9 J NUCL MATER JI J. Nucl. Mater. PD JAN PY 2013 VL 432 IS 1-3 BP 395 EP 406 DI 10.1016/j.jnucmat.2012.07.047 PG 12 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA 128XB UT WOS:000317801900052 ER PT J AU Egeland, GW Mariani, RD Hartmann, T Porter, DL Hayes, SL Kennedy, JR AF Egeland, G. W. Mariani, R. D. Hartmann, T. Porter, D. L. Hayes, S. L. Kennedy, J. R. TI Reducing fuel-cladding chemical interaction: The effect of palladium on the reactivity of neodymium on iron in diffusion couples SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID METALLIC FUEL; LATTICE-CONSTANTS; CRYSTAL-STRUCTURE; MINOR ACTINIDES; STAINLESS-STEEL; BARRIER; PERFORMANCE; FCCI; LANTHANIDES; BEHAVIOR AB Fast-reactor fuel alloys produce lanthanide fission products which migrate to the fuel/cladding interface causing fuel-cladding chemical interaction. To test viability of pinning these lanthanides, neodymium was selected as an iron interacting lanthanide and palladium was chosen as the dopant. An arc-melt produced 1:1 neodymium-palladium compound and pure neodymium were tested against iron in diffusion couples at temperatures above and below the Nd-Fe eutectic melting point. (c) 2012 Elsevier B.V. All rights reserved. C1 [Egeland, G. W.; Hartmann, T.] Univ Nevada, Harry Reid Ctr Environm Studies, Las Vegas, NV 89154 USA. [Mariani, R. D.; Porter, D. L.; Hayes, S. L.; Kennedy, J. R.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. RP Egeland, GW (reprint author), Univ Nevada, Harry Reid Ctr Environm Studies, Las Vegas, NV 89154 USA. EM gerald.egeland@gmail.com RI Hayes, Steven/D-8373-2017 OI Hayes, Steven/0000-0002-7583-2069 FU DOE [DE-AC07-05ID14517] FX We would like to thank Ariana Alaniz and Dr. Dan Koury for assistance at the Harry Reid Center for Environmental Studies at UNLV. This program was funded by DOE Contract No. DE-AC07-05ID14517. NR 21 TC 3 Z9 3 U1 0 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 J9 J NUCL MATER JI J. Nucl. Mater. PD JAN PY 2013 VL 432 IS 1-3 BP 539 EP 544 DI 10.1016/j.jnucmat.2012.07.028 PG 6 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA 128XB UT WOS:000317801900068 ER PT J AU Lawton, JS Jones, A Zawodzinski, T AF Lawton, Jamie S. Jones, Amanda Zawodzinski, Thomas TI Concentration Dependence of VO2+ Crossover of Nafion for Vanadium Redox Flow Batteries SO JOURNAL OF THE ELECTROCHEMICAL SOCIETY LA English DT Article ID ELECTRON-SPIN-RESONANCE; DIFFUSION-COEFFICIENTS; MEMBRANES; ION; TRANSPORT; WATER; MODEL; CONDUCTIVITY AB The VO2+ crossover,. or permeability, through Nafion in a vanadium redox flow battery (VRFB) was monitored as a function of sulfuric acid concentration and VO2+ concentration. A vanadium rich solution was flowed on one side of the membrane through a flow field while symmetrically on the other side a blank or vanadium deficit solution was flowed. The blank solution was flowed through an electron paramagnetic resonance (EPR) cavity and the VO2+ concentration was determined from the intensity of the EPR signal. Concentration values were fit using a solution of Fick's law that allows for the effect of concentration change on the vanadium rich side. The fits resulted in permeability values of VO2+ ions across the membrane. Viscosity measurements of many VO2+ and H2SO4 solutions were made at 30-60 degrees C. These viscosity values were then used to determine the effect of the viscosity of the flowing solution on the permeability of the ion. (C) 2013 The Electrochemical Society. [DOI: 10.1149/2.004306jes] All rights reserved. C1 [Lawton, Jamie S.; Jones, Amanda; Zawodzinski, Thomas] Univ Tennessee, Dept Chem & Biomol Engn, Knoxville, TN 37996 USA. [Zawodzinski, Thomas] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Lawton, JS (reprint author), Univ Tennessee, Dept Chem & Biomol Engn, Knoxville, TN 37996 USA. EM tzawodzi@utk.edu NR 27 TC 13 Z9 13 U1 7 U2 73 PU ELECTROCHEMICAL SOC INC PI PENNINGTON PA 65 SOUTH MAIN STREET, PENNINGTON, NJ 08534 USA SN 0013-4651 J9 J ELECTROCHEM SOC JI J. Electrochem. Soc. PY 2013 VL 160 IS 4 BP A697 EP A702 DI 10.1149/2.004306jes PG 6 WC Electrochemistry; Materials Science, Coatings & Films SC Electrochemistry; Materials Science GA 117TU UT WOS:000316976800025 ER PT J AU Sethuraman, VA Nguyen, A Chon, MJ Nadimpalli, SPV Wang, H Abraham, DP Bower, AF Shenoy, VB Guduru, PR AF Sethuraman, V. A. Nguyen, A. Chon, M. J. Nadimpalli, S. P. V. Wang, H. Abraham, D. P. Bower, A. F. Shenoy, V. B. Guduru, P. R. TI Stress Evolution in Composite Silicon Electrodes during Lithiation/Delithiation SO JOURNAL OF THE ELECTROCHEMICAL SOCIETY LA English DT Article ID LITHIUM-ION BATTERIES; SOLID-STATE AMORPHIZATION; IN-SITU MEASUREMENTS; NEGATIVE-ELECTRODES; HIGH-CAPACITY; ELECTROCHEMICAL PERFORMANCE; MECHANICAL-PROPERTIES; STRUCTURAL-CHANGES; POLYACRYLIC-ACID; CYCLE LIFE AB We report real-time average stress measurements on composite silicon electrodes made with two different binders viz. Carboxymethyl cellulose (CMC) and Polyvinylidene fluoride (PVDF) during electrochemical lithiation and delithiation. During galvanostatic lithiation at very slow rates, the stress in a CMC-based electrode becomes compressive and increases to 70 MPa, where it reaches a plateau and increases slowly thereafter with capacity. The PVDF-based electrode exhibits similar behavior, although with lower peak compressive stress of about 12 MPa. These initial experiments indicate that the stress evolution in a Si composite electrode depends strongly on the mechanical properties of the binder. Stress data obtained from a series of lithiation/delithiation cycles suggests plasticity induced irreversible shape changes in contacting Si particles, and as a result, the stress response of the system during any given lithiation/delithiation cycle depends on the cycling history of the electrode. While these results constitute the first in situ stress measurements on composite Si electrodes during electrochemical cycling, the diagnostic technique described herein can be used to assess the mechanical response of a composite electrode made with other active material/binder combinations. (C) 2013 The Electrochemical Society. [DOI: 10.1149/2.021306jes] All rights reserved. C1 [Sethuraman, V. A.; Nguyen, A.; Chon, M. J.; Nadimpalli, S. P. V.; Wang, H.; Bower, A. F.; Shenoy, V. B.; Guduru, P. R.] Brown Univ, Sch Engn, Providence, RI 02912 USA. [Abraham, D. P.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Shenoy, V. B.] Univ Penn, Dept Mat Sci & Engn, Philadelphia, PA 19104 USA. RP Sethuraman, VA (reprint author), Brown Univ, Sch Engn, Providence, RI 02912 USA. EM vj@cal.berkeley.edu; Pradeep_Guduru@Brown.edu RI Wang, Hailong/C-2330-2008; Sethuraman, Vijay/E-5702-2010; Nadimpalli, Siva/B-6777-2009; OI Sethuraman, Vijay/0000-0003-4624-1355; Nadimpalli, Siva/0000-0001-9281-4842 FU United States Department of Energy - EPSCoR Implementation award [DE-SC0007074] FX The authors gratefully acknowledge financial support from the United States Department of Energy - EPSCoR Implementation award (grant # DE-SC0007074). NR 47 TC 18 Z9 19 U1 4 U2 67 PU ELECTROCHEMICAL SOC INC PI PENNINGTON PA 65 SOUTH MAIN STREET, PENNINGTON, NJ 08534 USA SN 0013-4651 J9 J ELECTROCHEM SOC JI J. Electrochem. Soc. PY 2013 VL 160 IS 4 BP A739 EP A746 DI 10.1149/2.021306jes PG 8 WC Electrochemistry; Materials Science, Coatings & Films SC Electrochemistry; Materials Science GA 117TU UT WOS:000316976800032 ER PT J AU Xiao, N Li, N Cui, GF Tian, D Yu, SY Li, Q Wu, G AF Xiao, Ning Li, Ning Cui, Guofeng Tian, Dong Yu, Shiyou Li, Qing Wu, Gang TI Triblock Copolymers as Suppressors for Microvia Filling via Copper Electroplating SO JOURNAL OF THE ELECTROCHEMICAL SOCIETY LA English DT Article ID POLYETHYLENE-GLYCOL; PLATING FORMULA; CHLORIDE-IONS; PEG; ELECTRODEPOSITION; INHIBITION; BEHAVIOR; PPG; SPS; CL AB In this work, ethylene-propylene-ethylene (EPE) oxide triblock copolymers were found to be effective suppressors for microvia filling during copper electroplating. The studied EPE copolymers were divided into two groups according to their solubility and compositions. The first group was composed of EPE 1000, EPE 2000, and EPE 3500, and the second group contained EPE 2450, EPE 2900, and EPE 8000. In particular, the function of the triblock copolymer suppressors (e.g. EPE 2900) and their synergistic effect with other additives during copper electroplating were studied by galvanostatic measurements, suggesting that the suppression strength was greatly dependent on Cl-. In addition, cyclic voltammetry (CV) measurements indicated that a given suppressor in the plating bath required an optimal Cl- concentration to realize the strongest suppression strength. Then the filling performance of the plating bath using different suppressors was systematically compared by galvanostatic measurements and filling plating experiments in the plating bath with a fixed Cl- concentration (60 ppm), an optimal Cl- concentration, and a wide operation window of Cl- respectively. These experimental analyzes indicated that EPE 2000 and EPE 2900 were the best suppressors in the first and second group, respectively. The relevant mechanism of triblock copolymer suppressors for microvia filling was discussed. (C) 2013 The Electrochemical Society. [DOI: 10.1149/2.015306jes] All rights reserved. C1 [Xiao, Ning; Li, Ning; Tian, Dong; Yu, Shiyou] Harbin Inst Technol, Dept Appl Chem, Harbin 150001, Peoples R China. [Cui, Guofeng] Sun Yat Sen Univ, Sch Chem & Chem Engn, Guangzhou 510275, Guangdong, Peoples R China. [Li, Qing; Wu, Gang] Los Alamos Natl Lab, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA. RP Xiao, N (reprint author), Harbin Inst Technol, Dept Appl Chem, Harbin 150001, Peoples R China. EM lininghit@263.net RI Wu, Gang/E-8536-2010; Li, Qing/G-4502-2011 OI Wu, Gang/0000-0003-4956-5208; Li, Qing/0000-0003-4807-030X FU Highnic Group (China) FX This work was financially supported by Highnic Group (China). The authors gratefully acknowledge Sun He for her support to this work. NR 28 TC 8 Z9 8 U1 3 U2 39 PU ELECTROCHEMICAL SOC INC PI PENNINGTON PA 65 SOUTH MAIN STREET, PENNINGTON, NJ 08534 USA SN 0013-4651 J9 J ELECTROCHEM SOC JI J. Electrochem. Soc. PY 2013 VL 160 IS 4 BP D188 EP D195 DI 10.1149/2.015306jes PG 8 WC Electrochemistry; Materials Science, Coatings & Films SC Electrochemistry; Materials Science GA 117TU UT WOS:000316976800055 ER PT J AU Ahluwalia, RK Arisetty, S Wang, XP Wang, XH Subbaraman, R Ball, SC DeCrane, S Myers, DJ AF Ahluwalia, Rajesh K. Arisetty, Srikanth Wang, Xiaoping Wang, Xiaohua Subbaraman, Ram Ball, Sarah C. DeCrane, Stacy Myers, Deborah J. TI Thermodynamics and Kinetics of Platinum Dissolution from Carbon-Supported Electrocatalysts in Aqueous Media under Potentiostatic and Potentiodynamic Conditions SO JOURNAL OF THE ELECTROCHEMICAL SOCIETY LA English DT Article ID PROTON-EXCHANGE MEMBRANE; ELECTROLYTE FUEL-CELLS; PARTICLE-SIZE; ACID; DEGRADATION; DURABILITY; INSTABILITY; MECHANISM; TEM AB The stability of dispersed high surface area carbon-supported platinum nano-particle electrocatalysts (Pt/C) was investigated as a function of particle size (mean diameters of 1.9, 3.2, 7.1, and 12.7 nm) and oxide coverage under potentiostatic and potentiodynamic conditions in aqueous perchloric acid electrolyte. A non-ideal solid solution theory was formulated to explain the observed dependence of the equilibrium dissolved Pt concentration on potential, Pt particle size, and oxide coverage, as inferred from cyclic voltammetry measurements. The activities of Pt and PtOx in Pt-PtOx solid solutions were correlated with the oxide coverage and Pt particle size. The theoretical framework was also used to determine the rate constants for Pt dissolution and PtOx formation and reduction. The results from the kinetic model were found to be consistent with the measured Pt dissolution for triangle potential cycles with different upper and lower potential limits and scan rates. (C) 2013 The Electrochemical Society. [DOT: 10.1149/2.018306jes] All rights reserved. C1 [Ahluwalia, Rajesh K.; Arisetty, Srikanth; Wang, Xiaoping; Wang, Xiaohua; Subbaraman, Ram; DeCrane, Stacy; Myers, Deborah J.] Argonne Natl Lab, Argonne, IL 60439 USA. [Ball, Sarah C.] Johnson Matthey Technol Ctr, Reading RG4 9NH, Berks, England. [DeCrane, Stacy] Kettering Univ, Flint, MI 48503 USA. RP Ahluwalia, RK (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. EM walia@anl.gov FU Fuel Cell Technologies Office of the U.S. Department of Energy's (DOE) Office of Energy Efficiency and Renewable Energy; UChicago, Argonne, LLC [DE-AC02-06CH11357] FX This work was supported by the Fuel Cell Technologies Office of the U.S. Department of Energy's (DOE) Office of Energy Efficiency and Renewable Energy. Dr. Nancy Garland was the DOE technology development manager for this work. Argonne is a DOE, Office of Science Laboratory operated under Contract No. DE-AC02-06CH11357 by UChicago, Argonne, LLC. The authors thank the Analytical Chemistry Laboratory and Dr. Yifen Tsai at Argonne National Laboratory for the ICP-MS analyzes. The authors also thank Brian Theobald, Elvis Christian, and the Analytical Department at Johnson Matthey Technology Center for the preparation and TEM analysis of the catalyst materials. NR 30 TC 28 Z9 28 U1 1 U2 27 PU ELECTROCHEMICAL SOC INC PI PENNINGTON PA 65 SOUTH MAIN STREET, PENNINGTON, NJ 08534 USA SN 0013-4651 J9 J ELECTROCHEM SOC JI J. Electrochem. Soc. PY 2013 VL 160 IS 4 BP F447 EP F455 DI 10.1149/2.018306jes PG 9 WC Electrochemistry; Materials Science, Coatings & Films SC Electrochemistry; Materials Science GA 117TU UT WOS:000316976800078 ER PT J AU Gregoire, JM Xiang, C Mitrovic, S Liu, X Marcin, M Cornell, EW Fan, J Jin, J AF Gregoire, J. M. Xiang, C. Mitrovic, S. Liu, X. Marcin, M. Cornell, E. W. Fan, J. Jin, J. TI Combined Catalysis and Optical Screening for High Throughput Discovery of Solar Fuels Catalysts SO JOURNAL OF THE ELECTROCHEMICAL SOCIETY LA English DT Article ID WATER OXIDATION; MOLECULAR CATALYSTS; HYDROGEN-PRODUCTION; METAL-OXIDES AB Considerable research and development efforts are being devoted to the efficient generation of solar fuels. A solar fuels device couples a solar photoabsorber with catalysts to convert solar energy to chemical energy via reactions such as oxygen evolution (water splitting). Widespread deployment of this technology hinges upon discovery of new materials through efforts such as the high throughput screening of oxygen evolution catalysts, as discussed in this manuscript. We derive an expression for the efficiency of the oxygen evolution catalyst that combines catalytic and optical properties. Using this hybrid efficiency, we screen 5456 samples in a (Fe-Co-Ni-Ti)O-x. pseudo-quaternary catalyst library using automated, high throughput electrochemical and optical experiments. The observed compositional trends in this catalyst efficiency lead to the discovery of a new high performance composition region. (C) 2013 The Electrochemical Society. [DOI: 10.1149/2.035304jes] All rights reserved. C1 [Gregoire, J. M.; Xiang, C.; Mitrovic, S.; Liu, X.; Marcin, M.; Jin, J.] CALTECH, Joint Ctr Artificial Photosynth, Pasadena, CA 91125 USA. [Cornell, E. W.; Jin, J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Engn, Berkeley, CA 94720 USA. [Fan, J.] Zhejiang Univ, Dept Chem, Hangzhou 310027, Peoples R China. RP Gregoire, JM (reprint author), CALTECH, Joint Ctr Artificial Photosynth, Pasadena, CA 91125 USA. EM gregoire@caltech.edu RI Mitrovic, Slobodan/E-7847-2010 OI Mitrovic, Slobodan/0000-0001-8913-8505 FU Office of Science of the U.S. Department of Energy [DE-SC0004993]; National Science Foundation of China [21003106, 20873122] FX This material is based upon work performed by the Joint Center for Artificial Photosynthesis, a DOE Energy Innovation Hub, as follows: The experiments and data interpretation were supported through the Office of Science of the U.S. Department of Energy under Award No. DE-SC0004993; J.F. acknowledges financial support from the National Science Foundation of China (21003106 and 20873122). The authors thank Lung-Sheng Lin for assistance in fabrication of the cell and William Fisher of Lawrence Berkeley National Laboratory for assistance in fabrication of the capillary for the reference electrode. The authors also thank Dr. Joel Haber, Eric McFarland, Nathan Lewis, Carl Koval and Joachim Lewerenz for helpful discussions. NR 18 TC 29 Z9 29 U1 2 U2 44 PU ELECTROCHEMICAL SOC INC PI PENNINGTON PA 65 SOUTH MAIN STREET, PENNINGTON, NJ 08534 USA SN 0013-4651 J9 J ELECTROCHEM SOC JI J. Electrochem. Soc. PY 2013 VL 160 IS 4 BP F337 EP F342 DI 10.1149/2.035304jes PG 6 WC Electrochemistry; Materials Science, Coatings & Films SC Electrochemistry; Materials Science GA 117TU UT WOS:000316976800063 ER PT J AU Li, YH Gerdes, K Horita, T Liu, XB AF Li, Yihong Gerdes, Kirk Horita, Teruhisa Liu, Xingbo TI Surface Exchange and Bulk Diffusivity of LSCF as SOFC Cathode: Electrical Conductivity Relaxation and Isotope Exchange Characterizations SO JOURNAL OF THE ELECTROCHEMICAL SOCIETY LA English DT Article ID HIGH-TEMPERATURE PROPERTIES; CHEMICAL DIFFUSION; OXYGEN-TRANSPORT; ELECTRODE-KINETICS; CHARGE-TRANSFER; COEFFICIENT; LA0.6SR0.4CO0.2FE0.8O3-DELTA; REDUCTION; PATHWAYS; TRACER AB The oxygen diffusion coefficient (D) and surface exchange coefficient (k) of a typical SOFC cathode material, La0.6Sr0.4Ce0.2Fe0.5O3-delta (LSCF) were characterized by both electrical conductivity relaxation (ECR) and oxygen isotope exchange (IE) methods. Conductivity relaxation experiments were conducted at 800 degrees C for small step changes in partial pressure of oxygen (PO2), both decreasing and increasing, from 0.02 atm to 0.20 atm. The results revealed PO2 dependent hysteresis with the reduction process requiring more equilibration time than oxidation. Analysis of the experimental data indicated that the surface exchange coefficient is a function of the final oxygen partial pressure in an isothermal system. In addition, both forward and backward oxygen reduction reaction constants, which are vital for the fundamental understanding of SOFC cathode reaction mechanisms, are investigated based on the relationship between surface exchange coefficient and PO2. The direct comparisons between the results from both ECR and IE were presented and the possible experimental errors in both methods were discussed. (C) 2013 The Electrochemical Society. [DOI: 10.1149/2.044304jes] All rights reserved. C1 [Li, Yihong; Gerdes, Kirk; Liu, Xingbo] Natl Energy Technol Lab, Morgantown, WV 26507 USA. [Li, Yihong; Liu, Xingbo] W Virginia Univ, Dept Mech & Aerosp Engn, Morgantown, WV 26506 USA. [Horita, Teruhisa] Natl Inst Adv Ind Sci & Technol, Tsukuba, Ibaraki 3058565, Japan. RP Li, YH (reprint author), Natl Energy Technol Lab, Morgantown, WV 26507 USA. EM xingbo.liu@mail.wvu.edu FU National Energy Technology Laboratory in West Virginia University [DE-AC26-04NT41817] FX This technical effort from US was performed in support of the National Energy Technology Laboratory's on-going research in West Virginia University under contract #DE-AC26-04NT41817. The valuable technical assistance and discussion from Mingyang Gong and Greg Collins in WVU are acknowledged. The assistance of Richard Pineault, David Ruehl and Randall Gemmen from NETL in Morgantown, WV are highly appreciated. NR 37 TC 22 Z9 22 U1 4 U2 88 PU ELECTROCHEMICAL SOC INC PI PENNINGTON PA 65 SOUTH MAIN STREET, PENNINGTON, NJ 08534 USA SN 0013-4651 J9 J ELECTROCHEM SOC JI J. Electrochem. Soc. PY 2013 VL 160 IS 4 BP F343 EP F350 DI 10.1149/2.044304jes PG 8 WC Electrochemistry; Materials Science, Coatings & Films SC Electrochemistry; Materials Science GA 117TU UT WOS:000316976800064 ER PT J AU Olson, TS Dameron, AA Wood, K Pylpenko, S Hurst, KE Christensen, S Bult, JB Ginley, DS O'Hayre, R Dinh, H Gennett, T AF Olson, Tim S. Dameron, Arrelaine A. Wood, Kevin Pylpenko, Svitlana Hurst, Katherine E. Christensen, Steven Bult, Justin B. Ginley, David S. O'Hayre, Ryan Dinh, Huyen Gennett, Thomas TI Enhanced Fuel Cell Catalyst Durability with Nitrogen Modified Carbon Supports SO JOURNAL OF THE ELECTROCHEMICAL SOCIETY LA English DT Article ID PT-RU ALLOYS; METHANOL OXIDATION; PLATINUM NANOPARTICLES; DOPED CARBON; ELECTROOXIDATION; NANOTUBES; CROSSOVER AB This work illustrates the utility and improved performance of nitrogen-modified catalyst supports for direct methanol fuel cell (DMFC) applications. A unique two-step vapor-phase synthesis procedure is used to achieve the N-modification and Pt-Ru decoration of high surface-area carbon powders relevant to integration as electrocatalysts in fuel cell membrane electrode assemblies (MEA's). First, nitrogen surface moieties are incorporated into a commercial high surface area carbon support via a N-ion implantation technique, followed by Pt-Ru nanoparticle deposition via magnetron sputtering. The nitrogen-ion implantation of high surface area carbon supports yields superior Pt-Ru catalyst particle stability and performance as compared to industry standards. Specifically, results indicate a higher retention of metal catalyst surface area and electrochemical activity after accelerated electrochemical degradation testing. Further, characterization of catalyst materials before, during and after the electrochemical cycling provides insight into the catalyst particle coarsening and/or catalyst surface area loss mechanisms that dominate this fuel cell catalyst system. (C) 2013 The Electrochemical Society. [DOI: 10.1149/2.062304jes] All rights reserved. C1 [Olson, Tim S.; Dameron, Arrelaine A.; Hurst, Katherine E.; Christensen, Steven; Bult, Justin B.; Ginley, David S.; Dinh, Huyen; Gennett, Thomas] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Wood, Kevin; Pylpenko, Svitlana; O'Hayre, Ryan] Colorado Sch Mines, Golden, CO 80401 USA. RP Olson, TS (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM Thomas.Gennett@nrel.gov RI O'Hayre, Ryan/A-8183-2009 FU U.S. Department of Energy [DE-AC36-08-GO28308]; National Renewable Energy Laboratory; Army Research office [W911NF-09-1-0528] FX This work was supported by the U.S. Department of Energy under Contract No. DE-AC36-08-GO28308 with the National Renewable Energy Laboratory. The SAXS and XRD work on this project by the Colorado School of Mines was supported by the Army Research office (under Grant No. W911NF-09-1-0528). Portions of this research were carried out at the Stanford Synchrotron Radiation Lightsource (SSRL), a Directorate of SLAC National Accelerator Laboratory and an Office of Science User Facility operated for the U.S. Department of Energy Office of Science by Stanford University. We acknowledge Michael Toney, Tom Hostetler, Doug Van Campen, and John Pople for useful support regarding synchrotron experiments. NR 27 TC 12 Z9 12 U1 3 U2 42 PU ELECTROCHEMICAL SOC INC PI PENNINGTON PA 65 SOUTH MAIN STREET, PENNINGTON, NJ 08534 USA SN 0013-4651 J9 J ELECTROCHEM SOC JI J. Electrochem. Soc. PY 2013 VL 160 IS 4 BP F389 EP F394 DI 10.1149/2.062304jes PG 6 WC Electrochemistry; Materials Science, Coatings & Films SC Electrochemistry; Materials Science GA 117TU UT WOS:000316976800070 ER PT J AU Reifsnider, KL Chiu, WKS Brinkman, KS Du, YH Nakajo, A Rabbi, F Liu, QL AF Reifsnider, K. L. Chiu, Wilson K. S. Brinkman, Kyle S. Du, Yanhai Nakajo, Arata Rabbi, Fazle Liu, Qianlong TI Multiphysics Design and Development of Heterogeneous Functional Materials for Renewable Energy Devices: The HeteroFoaM Story SO JOURNAL OF THE ELECTROCHEMICAL SOCIETY LA English DT Article ID OXIDE FUEL-CELLS; X-RAY NANOTOMOGRAPHY; OXYGEN PERMEATION; THIN-FILMS; ION; COMPOSITE; CATHODES; ANODE; ELECTRODES; TRANSPORT AB The electrochemical science that makes many energy conversion and storage technologies work rests on our knowledge and understanding of heterogeneous materials and material systems. The function and functionality of those systems share many common features across a wide range of technologies including fuel cells; batteries, capacitors, and membranes. The science that controls that functionality for these complex material systems is typically summoned in fragments to design a specific device. The present paper discusses an attempt to create a codified multiphysics approach to that general subject, across multiple scales in space and time, for heterogeneous functional materials, or "HeteroFoaM" as we call it. The scope of the paper will be necessarily limited to a general definition of the problem focused on a few specific examples of the progress made for directions that support technologies such as conversion of chemical energy to electricity, membranes for selective transport, and charge storage devices. The principal motivation for this approach is to establish the science that controls emergent properties in heterogeneous functional materials as a foundation for design of functional material systems with performance not bounded by constituent properties. (C) 2013 The Electrochemical Society. [DOI: 10.1149/2.012306jes] All rights reserved. C1 [Reifsnider, K. L.; Du, Yanhai; Rabbi, Fazle; Liu, Qianlong] Univ S Carolina, Dept Mech Engn, Columbia, SC 29209 USA. [Chiu, Wilson K. S.; Nakajo, Arata] Univ Connecticut, Dept Mech Engn, Storrs, CT 06269 USA. [Brinkman, Kyle S.] Savannah River Natl Lab, Aiken, SC 29808 USA. RP Reifsnider, KL (reprint author), Univ S Carolina, Dept Mech Engn, Columbia, SC 29209 USA. EM Reifsnider@sc.edu OI Brinkman, Kyle/0000-0002-2219-1253 FU Energy Frontier Research Center for Heterogeneous Functional Materials, the HeteroFoaM Center under DoE from the Office of Basic Energy Sciences [DE-SC0001061]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357, DE-AC02-98CH10886]; Department of Energy [DE-AC09-08SR22470] FX This work was presented as a Keynote lecture at the symposium on "Renewable Fuels from Sunlight and Electricity," PRiME 2012/222nd Meeting of the Electrochemical Society, Honolulu, HI, October 7-12, 2012. The authors gratefully acknowledge the support of the Energy Frontier Research Center for Heterogeneous Functional Materials, the HeteroFoaM Center, for support of this research under DoE grant no. DE-SC0001061 from the Office of Basic Energy Sciences. The X-ray tomography elements of this research were carried out at the Advanced Photon Source (Dr. S. Wang) supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under contract No. DE-AC02-06CH11357, and at the National Synchrotron Light Source (Dr. J. Wang, Dr. K. Chen-Wiegart) at Brookhaven National Laboratory supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. SFM samples were provided by Prof. F. Chen (University of South Carolina) and Ni-YSZ samples were provided by MER Dr. J. Van herle (Ecole Polytechnique Federale de Lausanne, Switzerland). The oxygen membrane characterization elements of this research were carried out at the Savannah River National Laboratory (Dr. K. Brinkman) which operates under contract No. DE-AC09-08SR22470 with the Department of Energy. NR 67 TC 8 Z9 8 U1 0 U2 19 PU ELECTROCHEMICAL SOC INC PI PENNINGTON PA 65 SOUTH MAIN STREET, PENNINGTON, NJ 08534 USA SN 0013-4651 EI 1945-7111 J9 J ELECTROCHEM SOC JI J. Electrochem. Soc. PY 2013 VL 160 IS 4 BP F470 EP F481 DI 10.1149/2.012306jes PG 12 WC Electrochemistry; Materials Science, Coatings & Films SC Electrochemistry; Materials Science GA 117TU UT WOS:000316976800081 ER PT J AU Hatt, A AF Hatt, Alison TI Networking at the heart of African workshop on computational materials science SO MRS BULLETIN LA English DT Article RP Hatt, A (reprint author), Lawrence Berkeley Natl Lab, Berkeley, CA USA. RI Hatt, Alison/B-4652-2010 NR 0 TC 0 Z9 0 U1 0 U2 1 PU CAMBRIDGE UNIV PRESS PI NEW YORK PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA SN 0883-7694 J9 MRS BULL JI MRS Bull. PD JAN PY 2013 VL 38 IS 1 BP 12 EP 14 PG 3 WC Materials Science, Multidisciplinary; Physics, Applied SC Materials Science; Physics GA 125OP UT WOS:000317549400008 ER PT J AU French, WR Iacovella, CR Rungger, I Souza, AM Sanvito, S Cummings, PT AF French, William R. Iacovella, Christopher R. Rungger, Ivan Souza, Amaury Melo Sanvito, Stefano Cummings, Peter T. TI Atomistic simulations of highly conductive molecular transport junctions under realistic conditions SO NANOSCALE LA English DT Article ID GOLD NANOWIRES; BENZENEDITHIOL; ELONGATION; DYNAMICS; MECHANISM; GEOMETRY; ATOMS AB We report state-of-the-art atomistic simulations combined with high-fidelity conductance calculations to probe structure-conductance relationships in Au-benzenedithiolate (BDT)-Au junctions under elongation. Our results demonstrate that large increases in conductance are associated with the formation of monatomic chains (MACs) of Au atoms directly connected to BDT. An analysis of the electronic structure of the simulated junctions reveals that enhancement in the s-like states in Au MACs causes the increases in conductance. Other structures also result in increased conductance but are too short-lived to be detected in experiment, while MACs remain stable for long simulation times. Examinations of thermally evolved junctions with and without MACs show negligible overlap between conductance histograms, indicating that the increase in conductance is related to this unique structural change and not thermal fluctuation. These results, which provide an excellent explanation for a recently observed anomalous experimental result [Bruot et al., Nat. Nanotechnol., 2012, 7, 35-40], should aid in the development of mechanically responsive molecular electronic devices. C1 [French, William R.; Iacovella, Christopher R.; Cummings, Peter T.] Dept Chem & Biomol Engn, Nashville, TN USA. [Rungger, Ivan; Souza, Amaury Melo; Sanvito, Stefano] Trinity Coll Dublin, Sch Phys, Dublin 2, Ireland. [Rungger, Ivan; Souza, Amaury Melo; Sanvito, Stefano] Trinity Coll Dublin, CRANN, Dublin 2, Ireland. [Cummings, Peter T.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN USA. RP Cummings, PT (reprint author), Dept Chem & Biomol Engn, Nashville, TN USA. EM peter.cummings@vanderbilt.edu RI Iacovella, Christopher/D-2050-2011; French, William/D-4164-2013; Souza, Amaury/H-9474-2014 OI French, William/0000-0003-2927-0234; FU U.S. Department of Education for a Graduate Assistance in Areas of National Need (GAANN) Fellowship [P200A090323]; National Science Foundation [CBET-1028374]; King Abdullah University of Science and Technology (ACRAB project); National Energy Research Scientific Computing Center (NERSC); Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX WRF acknowledges partial support from the U.S. Department of Education for a Graduate Assistance in Areas of National Need (GAANN) Fellowship under grant number P200A090323; WRF, CRI and PTC acknowledge partial support from the National Science Foundation through grant CBET-1028374. IR, AMS, and SS thank the King Abdullah University of Science and Technology (ACRAB project) for financial support. This research used resources of the National Energy Research Scientific Computing Center (NERSC), which is supported by the Office of Science of the U.S. Department of Energy under Contract no. DE-AC02-05CH11231; specifically, the conductance calculations were performed on NERSC's Carver. NR 43 TC 17 Z9 17 U1 4 U2 35 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2040-3364 J9 NANOSCALE JI Nanoscale PY 2013 VL 5 IS 9 BP 3654 EP 3659 DI 10.1039/c3nr00459g PG 6 WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 129RK UT WOS:000317859400012 PM 23552959 ER PT J AU Schlung, SA Ravelo, AC Aiello, IW Andreasen, DH Cook, MS Drake, M Dyez, KA Guilderson, TP LaRiviere, JP Stroynowski, Z Takahashi, K AF Schlung, Shiloh A. Ravelo, A. Christina Aiello, Ivano W. Andreasen, Dyke H. Cook, Mea S. Drake, Michelle Dyez, Kelsey A. Guilderson, Thomas P. LaRiviere, Jonathan P. Stroynowski, Zuzanna Takahashi, Kozo TI Millennial-scale climate change and intermediate water circulation in the Bering Sea from 90 ka: A high-resolution record from IODP Site U1340 SO PALEOCEANOGRAPHY LA English DT Article ID SANTA-BARBARA BASIN; SUB-ARCTIC PACIFIC; LAST GLACIAL TERMINATION; OXYGEN-MINIMUM ZONE; YOUNGER DRYAS EVENT; NORTH PACIFIC; NORTHWESTERN PACIFIC; CYCLADOPHORA-DAVISIANA; OCEAN CIRCULATION; HEINRICH EVENT-1 AB Millennial-scale climate events in the North Pacific are thought to be related to changes in the circulation of North Pacific Intermediate Water, which may have formed in the Bering Sea in the past. To advance our understanding of the mechanisms that underlie millennial-scale events, Bering Sea sediment cores from the Integrated Ocean Drilling Program site U1340 were used to construct high-resolution, multiproxy climate records of the last 90,000 years. Sediment density records show millennial-scale events resembling Dansgaard-Oeschger events, several of which are laminated. Interstadials were characterized by 3-5 degrees C warming, increased productivity driven by upwelling, and reduced benthic oxygenation. Bering Sea intermediate water also changed over longer timescales; our records show the presence of intermediate water with lower salinity and higher oxygen content than modern beginning around 60 ka and persisting until the beginning of the deglaciation. The Bolling-Allerod was characterized by high productivity, laminated sediments, and strong denitrification signature. Our data support the idea that productivity-derived changes in oxygenation at intermediate water source regions may have contributed to the intensification of the North Pacific-wide oxygen minima during the Bolling-Allerod. Citation: Schlung, S. A., A. Christina Ravelo, I. W. Aiello, D. H. Andreasen, M. S. Cook, M. Drake, K. A. Dyez, T. P. Guilderson, J. P. LaRiviere, Z. Stroynowski, and K. Takahashi (2013), Millennial-scale climate change and intermediate water circulation in the Bering Sea from 90 ka: A high-resolution record from IODP Site U1340, Paleoceanography, 28, 54-67, doi:10.1029/2012PA002365. C1 [Schlung, Shiloh A.; Ravelo, A. Christina; Guilderson, Thomas P.; LaRiviere, Jonathan P.; Stroynowski, Zuzanna] Univ Calif Santa Cruz, Ocean Sci Dept, Santa Cruz, CA 95064 USA. [Aiello, Ivano W.; Drake, Michelle] Moss Landing Marine Labs, Moss Landing, CA 95039 USA. [Andreasen, Dyke H.; Dyez, Kelsey A.] Williams Coll, Williamstown, MA 01267 USA. [Cook, Mea S.] Lawrence Livermore Natl Lab, Ctr Accelerator Mass Spectrometry, Livermore, CA 94551 USA. [Guilderson, Thomas P.] Univ Calif Santa Cruz, Earth & Planetary Sci Dept, Santa Cruz, CA 95064 USA. [Takahashi, Kozo] Hokusei Gakuen Univ, Atsubetsu Ku, Sapporo, Hokkaido 0048631, Japan. RP Ravelo, AC (reprint author), Univ Calif Santa Cruz, Ocean Sci Dept, 1156 High St, Santa Cruz, CA 95064 USA. EM acr@ucsc.edu FU National Science Foundation [OCE0963144]; Consortium for Ocean Leadership [T323A7-001] FX The authors thank the IODP and all the crew, staff, technicians, and scientists on the JOIDES Resolution during IODP Expedition 323 to the Bering Sea. They also thank Elektra Robinson and Michaela Gwiazda for their help with sample preparation. This work was funded by the National Science Foundation (grant no. OCE0963144) and the Consortium for Ocean Leadership (award no. T323A7-001). NR 104 TC 13 Z9 14 U1 1 U2 43 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0883-8305 EI 1944-9186 J9 PALEOCEANOGRAPHY JI Paleoceanography PY 2013 VL 28 IS 1 DI 10.1029/2012PA002365 PG 14 WC Geosciences, Multidisciplinary; Oceanography; Paleontology SC Geology; Oceanography; Paleontology GA 129KO UT WOS:000317838200006 ER PT J AU Baalrud, SD AF Baalrud, S. D. TI The incomplete plasma dispersion function: Properties and application to waves in bounded plasmas SO PHYSICS OF PLASMAS LA English DT Article ID MAXWELLIAN VELOCITY DISTRIBUTION; ELECTRONIC LONGITUDINAL MODES; LASER-INDUCED FLUORESCENCE; ELECTROSTATIC OSCILLATIONS; CUTOFF DISTRIBUTIONS; 2-POLE APPROXIMATION; LOW-PRESSURE; DOUBLE-LAYER; PROPAGATION; PERTURBATIONS AB The incomplete plasma dispersion function is a generalization of the plasma dispersion function in which the defining integral spans a semi-infinite, rather than infinite, domain. It is useful for describing the linear dielectric response and wave dispersion in non-Maxwellian plasmas when the distribution functions can be approximated as Maxwellian over finite, or semi-infinite, intervals in velocity phase-space. A ubiquitous example is the depleted Maxwellian electron distribution found near boundary sheaths or double layers, where the passing interval can be modeled as Maxwellian with a lower temperature than the trapped interval. The depleted Maxwellian is used as an example to demonstrate the utility of using the incomplete plasma dispersion function for calculating modifications to wave dispersion relations. (C) 2013 American Institute of Physics. [http://dx.doi.org/10.1063/1.4789387] C1 [Baalrud, S. D.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Baalrud, S. D.] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. RP Baalrud, SD (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. FU National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396]; U.S. Department of Energy Fusion Energy Postdoctoral Research Program FX The author thanks Professor F. Skiff for reading and commenting on the manuscript and Professor C. C. Hegna for helpful discussions. This research was supported in part by an appointment to the U.S. Department of Energy Fusion Energy Postdoctoral Research Program administered by the Oak Ridge Institute for Science and Education, and in part under the auspices of the National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396. NR 55 TC 1 Z9 1 U1 1 U2 14 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 1070-664X J9 PHYS PLASMAS JI Phys. Plasmas PD JAN PY 2013 VL 20 IS 1 AR 012118 DI 10.1063/1.4789387 PG 13 WC Physics, Fluids & Plasmas SC Physics GA 122AC UT WOS:000317286200020 ER PT J AU Bellei, C Amendt, PA Wilks, SC Haines, MG Casey, DT Li, CK Petrasso, R Welch, DR AF Bellei, C. Amendt, P. A. Wilks, S. C. Haines, M. G. Casey, D. T. Li, C. K. Petrasso, R. Welch, D. R. TI Species separation in inertial confinement fusion fuels SO PHYSICS OF PLASMAS LA English DT Article ID NATIONAL IGNITION FACILITY; SHOCK-WAVE; MIXTURES; TARGETS AB It is shown by means of multi-fluid particle-in-cell simulations that convergence of the spherical shock wave that propagates through the inner gas of inertial confinement fusion-relevant experiments is accompanied by a separation of deuterium (D) and tritium (T) ions across the shock front. Deuterons run ahead of the tritons due to their lower mass and higher charge-to-mass ratio and can reach the center several tens of picoseconds before the tritons. The rising edge of the DD and TT fusion rate is also temporally separated by the same amount, which should be an observable in experiments and would be a direct proof of the "stratification conjecture" on the shock front [Amendt et al., Phys. Plasmas 18, 056308 (2011)]. Moreover, dephasing of the D and T shock components in terms of density and temperature leads to a degradation of the DT fusion yield as the converging shock first rebounds from the fuel center (shock yield). For the parameters of this study, the second peak in the fusion yield (compression yield) is strongly dependent on the choice of the flux limiter. (C) 2013 American Institute of Physics. [http://dx.doi.org/10.1063/1.4773291] C1 [Bellei, C.; Amendt, P. A.; Wilks, S. C.; Casey, D. T.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Haines, M. G.] Univ London Imperial Coll Sci Technol & Med, Blackett Lab, London SW7 2AZ, England. [Casey, D. T.; Li, C. K.; Petrasso, R.] MIT, Plasma Sci & Fus Ctr, Cambridge, MA 02139 USA. [Welch, D. R.] Voss Scient, Albuquerque, NM 87108 USA. RP Bellei, C (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. FU LLNL Computational Directorate Grand Challenge award; U.S. Department of Energy [DE-AC52-07NA27344]; [LDRD-11-ERD-075] FX Useful discussions with D. Ryutov and E. Williams are acknowledged. The authors also thank P. B. Radha for providing Lilac simulation results. Computing support for this work came from a LLNL Computational Directorate Grand Challenge award.; This work was performed under the auspices of the U.S. Department of Energy by the Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344 and supported by LDRD-11-ERD-075. NR 25 TC 22 Z9 22 U1 1 U2 26 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 1070-664X J9 PHYS PLASMAS JI Phys. Plasmas PD JAN PY 2013 VL 20 IS 1 AR 012701 DI 10.1063/1.4773291 PG 8 WC Physics, Fluids & Plasmas SC Physics GA 122AC UT WOS:000317286200052 ER PT J AU Black, C Germaschewski, K Bhattacharjee, A Ng, CS AF Black, Carrie Germaschewski, Kai Bhattacharjee, Amitava Ng, C. S. TI Discrete kinetic eigenmode spectra of electron plasma oscillations in weakly collisional plasma: A numerical study SO PHYSICS OF PLASMAS LA English DT Article ID FOKKER-PLANCK EQUATION; VLASOV EQUATION; VELOCITY SPACE; INTEGRATION; DIFFUSION; MODES AB It has been demonstrated that in the presence of weak collisions, described by the Lenard-Bernstein (LB) collision operator, the Landau-damped solutions become true eigenmodes of the system and constitute a complete set [C.-S. Ng et al., Phys. Rev. Lett. 83, 1974 (1999) and C. S. Ng et al., Phys. Rev. Lett. 96, 065002 (2004)]. We present numerical results from an Eulerian Vlasov code that incorporates the Lenard-Bernstein collision operator [A. Lenard and I. B. Bernstein, Phys. Rev. 112, 1456 (1958)]. The effect of collisions on the numerical recursion phenomenon seen in Vlasov codes is discussed. The code is benchmarked against exact linear eigenmode solutions in the presence of weak collisions, and a spectrum of Landau-damped solutions is determined within the limits of numerical resolution. Tests of the orthogonality and the completeness relation are presented. (C) 2013 American Institute of Physics. [http://dx.doi.org/10.1063/1.4789882] C1 [Black, Carrie] NASA, Goddard Space Flight Ctr, Space Weather Lab, Greenbelt, MD 20771 USA. [Germaschewski, Kai; Bhattacharjee, Amitava] Univ New Hampshire, Dept Phys, Ctr Integrated Computat & Anal Reconnect & Turbul, Inst Study Earth Oceans & Space, Durham, NH 03824 USA. [Ng, C. S.] Univ Alaska, Inst Geophys, Fairbanks, AK 99775 USA. [Ng, C. S.] Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. RP Black, C (reprint author), NASA, Goddard Space Flight Ctr, Space Weather Lab, Greenbelt, MD 20771 USA. EM Carrie.Black@nasa.gov RI Ng, Chung-Sang/F-2980-2011 OI Ng, Chung-Sang/0000-0003-1861-5356 FU NSF [CNS-0855145, AGS-1056898]; DOE [ER55093]; National Science Foundation [PHY-1004357]; National Science Foundation of China NSFC [41128004] FX This work was conducted at the Center for Integrated Computation and Analysis of Reconnection and Turbulence (CICART) at the Institute for the Study of Earth, Oceans, and Space located at the University of New Hampshire. The research of C.B. is supported by an appointment to the NASA Postdoctoral Program at the Goddard Space Flight Center, administered by Oak Ridge Associated Universities through a contract with NASA. K.G. is supported by NSF Grants CNS-0855145 and AGS-1056898 and DOE Grant ER55093. C.S.N. is supported in part by a National Science Foundation Grant PHY-1004357 and by the National Science Foundation of China NSFC under Grant No. 41128004. NR 21 TC 2 Z9 2 U1 0 U2 8 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD JAN PY 2013 VL 20 IS 1 AR 012125 DI 10.1063/1.4789882 PG 10 WC Physics, Fluids & Plasmas SC Physics GA 122AC UT WOS:000317286200027 ER PT J AU Burby, JW Qin, H AF Burby, J. W. Qin, H. TI Toroidal precession as a geometric phase SO PHYSICS OF PLASMAS LA English DT Article ID GUIDING-CENTER MOTION; PARTICLES; STABILIZATION; TOKAMAKS; IONS AB Toroidal precession is commonly understood as the orbit-averaged toroidal drift of guiding centers in axisymmetric and quasisymmetric configurations. We give a new, more natural description of precession as a geometric phase effect. In particular, we show that the precession angle arises as the holonomy of a guiding center's poloidal trajectory relative to a principal connection. The fact that this description is physically appropriate is borne out with new, manifestly coordinate-independent expressions for the precession angle that apply to all types of orbits in tokamaks and quasisymmetric stellarators alike. We then describe how these expressions may be fruitfully employed in numerical calculations of precession. (C) 2013 American Institute of Physics. [http://dx.doi.org/10.1063/1.4789377] C1 [Burby, J. W.; Qin, H.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. [Qin, H.] Univ Sci & Technol China, Dept Modern Phys, Hefei 230026, Anhui, Peoples R China. RP Burby, JW (reprint author), Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA. FU U.S. Department of Energy [DE-AC02-09CH11466] FX We would like to thank Roscoe White, Nik Logan, and Jack Berkery for several illuminating conversations. We would also like to express our appreciation to Ben Faber and Jeff Parker for proof reading early versions of this manuscript. Finally, we are especially grateful to Jordan T. Burby for creating the figures that appear in the text. This work was supported by the U.S. Department of Energy under Contract No. DE-AC02-09CH11466. NR 29 TC 1 Z9 1 U1 5 U2 20 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 1070-664X J9 PHYS PLASMAS JI Phys. Plasmas PD JAN PY 2013 VL 20 IS 1 AR 012511 DI 10.1063/1.4789377 PG 10 WC Physics, Fluids & Plasmas SC Physics GA 122AC UT WOS:000317286200047 ER PT J AU Chen, H Sheppard, JC Meyerhofer, DD Hazi, A Link, A Anderson, S Baldis, HA Fedosejev, R Gronberg, J Izumi, N Kerr, S Marley, E Park, J Tommasini, R Wilks, S Williams, GJ AF Chen, Hui Sheppard, J. C. Meyerhofer, D. D. Hazi, A. Link, A. Anderson, S. Baldis, H. A. Fedosejev, R. Gronberg, J. Izumi, N. Kerr, S. Marley, E. Park, J. Tommasini, R. Wilks, S. Williams, G. J. TI Emittance of positron beams produced in intense laser plasma interaction SO PHYSICS OF PLASMAS LA English DT Article AB The first measurement of the emittance of intense laser-produced positron beams has been made. The emittance values were derived through measurements of positron beam divergence and source size for different peak positron energies under various laser conditions. For one of these laser conditions, we used a one dimensional pepper-pot technique to refine the emittance value. The laser-produced positrons have a geometric emittance between 100 and 500mm.mrad, comparable to the positron sources used at existing accelerators. With 10(10)-10(12) positrons per bunch, this low emittance beam, which is quasi-monoenergetic in the energy range of 5-20 MeV, may be useful as an alternative positron source for future accelerators. (C) 2013 American Institute of Physics. [http://dx.doi.org/10.1063/1.4789621] C1 [Chen, Hui; Hazi, A.; Link, A.; Anderson, S.; Gronberg, J.; Izumi, N.; Tommasini, R.; Wilks, S.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Sheppard, J. C.] Standford Univ, SLAC, Menlo Pk, CA 94025 USA. [Meyerhofer, D. D.] Univ Rochester, Laser Energet Lab, Rochester, NY 14623 USA. [Baldis, H. A.; Marley, E.; Park, J.; Williams, G. J.] Univ Calif Davis, Dept Elect & Comp Engn, Davis, CA 95616 USA. [Fedosejev, R.; Kerr, S.] Univ Alberta, Dept Appl Sci, Edmonton, AB T6G 2R3, Canada. RP Chen, H (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RI IZUMI, Nobuhiko/J-8487-2016; Tommasini, Riccardo/A-8214-2009; OI IZUMI, Nobuhiko/0000-0003-1114-597X; Tommasini, Riccardo/0000-0002-1070-3565; Kerr, Shaun/0000-0003-4822-564X FU U.S. DOE by LLNL [DE-AC52-07NA27344]; LLNL LDRD program FX We thank Dr. Tor Raubenheimer (SLAC) for initiating this work, Dr. Aaron Tremaine for discussion, and Dr. Peter Beiersdorfer, Dr. Bob Cauble, Dr. Henry Shaw, and Dr. Bill Goldstein for their encouragement and support. We gratefully acknowledge the JLF and Omega EP facility support during the experiment. This work was performed under the auspices of the U.S. DOE by LLNL under Contract No. DE-AC52-07NA27344, the computation was supported by LLNL Grand Computing Challenge time-allocation. The work was funded by the LLNL LDRD program. NR 35 TC 14 Z9 15 U1 2 U2 20 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD JAN PY 2013 VL 20 IS 1 AR 013111 DI 10.1063/1.4789621 PG 5 WC Physics, Fluids & Plasmas SC Physics GA 122AC UT WOS:000317286200070 ER PT J AU Chen, Y Munsat, T Parker, SE Heidbrink, WW Van Zeeland, MA Tobias, BJ Domier, CW AF Chen, Y. Munsat, T. Parker, S. E. Heidbrink, W. W. Van Zeeland, M. A. Tobias, B. J. Domier, C. W. TI Gyrokinetic simulations of reverse shear Alfven eigenmodes in DIII-D plasmas SO PHYSICS OF PLASMAS LA English DT Article ID DRIVEN AB A gyrokinetic ion/mass-less fluid electron hybrid model as implemented in the GEM code [Y. Chen and S. E. Parker, J. Comput. Phys. 220, 837 (2007)] is used to study the reverse shear Alfven eigenmodes (RSAE) observed in DIII-D, discharge #142111. This is a well diagnosed case with measurement of the core-localized RSAE mode structures and the mode frequency, which can be used to compare with simulations. Simulations reproduce many features of the observation, including the mode frequency up-sweeping in time and the sweeping range. A new algorithmic feature is added to the GEM code for this study. Instead of the gyrokinetic Poisson equation itself, its time derivative, or the vorticity equation, is solved to obtain the electric potential. This permits a numerical scheme that ensures the E x B convection of the equilibrium density profiles of each species cancel each other in the absence of any finite-Larmor-radius effects. These nonlinear simulations generally result in an electron temperature fluctuation level that is comparable to measurements, and a mode frequency spectrum broader than the experimental spectrum. The spectral width from simulations can be reduced if less steep beam density profiles are used, but then the experimental fluctuation level can be reproduced only if a collision rate above the classical level is assumed. (C) 2013 American Institute of Physics. [http://dx.doi.org/10.1063/1.4775776] C1 [Chen, Y.; Munsat, T.; Parker, S. E.] Univ Colorado, Boulder, CO 80309 USA. [Heidbrink, W. W.] Univ Calif Irvine, Irvine, CA 92697 USA. [Van Zeeland, M. A.] Gen Atom Co, San Diego, CA 92186 USA. [Tobias, B. J.] Princeton Plasma Phys Lab, Princeton, NJ 08540 USA. [Domier, C. W.] Univ Calif Davis, Davis, CA 95616 USA. RP Chen, Y (reprint author), Univ Colorado, Boulder, CO 80309 USA. FU U.S. Department of Energy's SciDAC project "Center for Nonlinear Simulation of Energetic Particles in Burning Plasmas"; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX The authors thank Dr. Guo-Yong Fu for helpful discussions. This work was supported by the U.S. Department of Energy's SciDAC project "Center for Nonlinear Simulation of Energetic Particles in Burning Plasmas." This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 25 TC 13 Z9 13 U1 3 U2 9 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 1070-664X J9 PHYS PLASMAS JI Phys. Plasmas PD JAN PY 2013 VL 20 IS 1 AR 012109 DI 10.1063/1.4775776 PG 11 WC Physics, Fluids & Plasmas SC Physics GA 122AC UT WOS:000317286200011 ER PT J AU Diallo, A Kramer, GJ Smith, DR Maingi, R Bell, RE Guttenfelder, W LeBlanc, BP Podesta, M McKee, GJ Fonck, R AF Diallo, A. Kramer, G. J. Smith, D. R. Maingi, R. Bell, R. E. Guttenfelder, W. LeBlanc, B. P. Podesta, M. McKee, G. J. Fonck, R. TI Observation of ion scale fluctuations in the pedestal region during the edge-localized-mode cycle on the National Spherical Torus Experiment SO PHYSICS OF PLASMAS LA English DT Article ID CORRELATION REFLECTOMETRY; FUSION PLASMAS; MICROWAVE REFLECTOMETRY; NSTX; TURBULENCE; ELM AB Characterization of the spatial structure of turbulence fluctuations during the edge localized mode cycle in the pedestal region is reported. Using the beam emission spectroscopy and the correlation reflectometry systems, measurements show spatial structure-k(perpendicular to)rho(ped)(i)-ranging from 0.2 to 0.7 propagating in the ion diamagnetic drift direction at the pedestal top. These propagating spatial scales are found to be anisotropic and consistent with ion-scale microturbulence of the type ion temperature gradient and/or kinetic ballooning modes. (C) 2013 American Institute of Physics. [http://dx.doi.org/10.1063/1.4773402] C1 [Diallo, A.; Kramer, G. J.; Bell, R. E.; Guttenfelder, W.; LeBlanc, B. P.; Podesta, M.; Fonck, R.] Princeton Plasma Phys Lab, Princeton, NJ 08540 USA. [Smith, D. R.; McKee, G. J.; Fonck, R.] Univ Wisconsin, Dept Engn Phys, Madison, WI USA. [Smith, D. R.; McKee, G. J.; Fonck, R.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Maingi, R.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Diallo, A (reprint author), Princeton Plasma Phys Lab, Princeton, NJ 08540 USA. RI Diallo, Ahmed/M-7792-2013 FU U.S. Department of Energy [DE-AC0209CH11466] FX The NSTX team is gratefully acknowledged. We thank the UCLA group for providing the data. A. D. acknowledges T. Osborne for providing the python tools for profile analysis, and J. Menard, S. Kaye, J. Manickam, and C. S. Chang for useful discussions. This manuscript has been authored by Princeton University and collaborators supported by U.S. Department of Energy Contract DE-AC0209CH11466. NR 43 TC 9 Z9 9 U1 0 U2 12 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 1070-664X J9 PHYS PLASMAS JI Phys. Plasmas PD JAN PY 2013 VL 20 IS 1 AR 012505 DI 10.1063/1.4773402 PG 8 WC Physics, Fluids & Plasmas SC Physics GA 122AC UT WOS:000317286200041 ER PT J AU Dorf, MA Cohen, RH Dorr, M Rognlien, T Hittinger, J Compton, J Colella, P Martin, D McCorquodale, P AF Dorf, M. A. Cohen, R. H. Dorr, M. Rognlien, T. Hittinger, J. Compton, J. Colella, P. Martin, D. McCorquodale, P. TI Simulation of neoclassical transport with the continuum gyrokinetic code COGENT SO PHYSICS OF PLASMAS LA English DT Article ID FINITE ASPECT RATIO; ARBITRARY COLLISIONALITY; PARTICLE SIMULATION; ELECTRIC-FIELD; PLASMAS; TURBULENCE; OPERATOR; PROGRESS; SYSTEMS; REGIME AB The development of the continuum gyrokinetic code COGENT for edge plasma simulations is reported. The present version of the code models a nonlinear axisymmetric 4D (R, v(parallel to), mu) gyrokinetic equation coupled to the long-wavelength limit of the gyro-Poisson equation. Here, R is the particle gyrocenter coordinate in the poloidal plane, and v(parallel to) and mu are the guiding center velocity parallel to the magnetic field and the magnetic moment, respectively. The COGENT code utilizes a fourth-order finite-volume (conservative) discretization combined with arbitrary mapped multiblock grid technology (nearly field-aligned on blocks) to handle the complexity of tokamak divertor geometry with high accuracy. Topics presented are the implementation of increasingly detailed model collision operators, and the results of neoclassical transport simulations including the effects of a strong radial electric field characteristic of a tokamak pedestal under H-mode conditions. (C) 2013 American Institute of Physics. [http://dx.doi.org/10.1063/1.4776712] C1 [Dorf, M. A.; Cohen, R. H.; Dorr, M.; Rognlien, T.; Hittinger, J.; Compton, J.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Colella, P.; Martin, D.; McCorquodale, P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Dorf, MA (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. FU U.S. Department of Energy [DE-AC52-07NA27344] FX The authors are grateful to B. Cohen, I. Joseph, M. Umansky, and X. Xu for fruitful discussions. This research was supported by the U.S. Department of Energy under contract DE-AC52-07NA27344. NR 49 TC 7 Z9 7 U1 2 U2 15 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 1070-664X J9 PHYS PLASMAS JI Phys. Plasmas PD JAN PY 2013 VL 20 IS 1 AR 012513 DI 10.1063/1.4776712 PG 13 WC Physics, Fluids & Plasmas SC Physics GA 122AC UT WOS:000317286200049 ER PT J AU Doss, FW Loomis, EN Welser-Sherrill, L Fincke, JR Flippo, KA Keiter, PA AF Doss, F. W. Loomis, E. N. Welser-Sherrill, L. Fincke, J. R. Flippo, K. A. Keiter, P. A. TI Instability, mixing, and transition to turbulence in a laser-driven counterflowing shear experiment SO PHYSICS OF PLASMAS LA English DT Article ID LAYERS; COMPRESSIBILITY AB In a turbulence experiment conducted at the Omega Laser Facility [Boehly et al., Opt. Commun. 133, 495 (1997)]], regions of 60 mg/cc foam are separated by an aluminum plate running the length of a 1.6mm shock tube. Two counter-propagating laser-driven shocks are used to create a high speed, Delta V 140 km/s shear flow environment, sustained for similar to 10 ns, while canceling the transverse pressure gradient across the interface. The spreading of the aluminum by shear-instability-induced mixing is measured by x-ray radiography. The width of the mix region is compared to simulations. Reynolds numbers greater than or similar to 4 x 10(5) are achieved within the layer. Following the onset of shear, we observe striations corresponding to the dominant mode growth and their transition through non-linear structures to developed turbulence. (C) 2013 American Institute of Physics. [http://dx.doi.org/10.1063/1.4789618] C1 [Doss, F. W.; Loomis, E. N.; Welser-Sherrill, L.; Fincke, J. R.; Flippo, K. A.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Keiter, P. A.] Univ Michigan, Dept Atmospher Ocean & Space Sci, Ann Arbor, MI 48109 USA. RP Doss, FW (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM fdoss@lanl.gov RI Keiter, Paul/J-3037-2013; Flippo, Kirk/C-6872-2009 OI Flippo, Kirk/0000-0002-4752-5141 FU U.S. Department of Energy; [DE-AC52-06NA25396] FX The authors are grateful to the LANL MST-7 target fabrication and P-24 operations teams. This work was supported by the U.S. Department of Energy and operated by Los Alamos National Security LLC under Contract No. DE-AC52-06NA25396. NR 23 TC 14 Z9 14 U1 2 U2 15 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD JAN PY 2013 VL 20 IS 1 AR 012707 DI 10.1063/1.4789618 PG 8 WC Physics, Fluids & Plasmas SC Physics GA 122AC UT WOS:000317286200058 ER PT J AU Ellison, CL Matyash, K Parker, JB Raitses, Y Fisch, NJ AF Ellison, C. L. Matyash, K. Parker, J. B. Raitses, Y. Fisch, N. J. TI Comment on "Three-dimensional numerical investigation of electron transport with rotating spoke in a cylindrical anode layer Hall plasma accelerator" [Phys. Plasmas 19, 073519 (2012)] SO PHYSICS OF PLASMAS LA English DT Editorial Material ID THRUSTERS; OSCILLATIONS; DISCHARGE AB The oscillation behavior described by Tang et al. [Phys. Plasmas 19, 073519 (2012)] differs too greatly from previous experimental and numerical studies to claim observation of the same phenomenon. Most significantly, the rotation velocity by Tang et al. [Phys. Plasmas 19, 073519 (2012)] is three orders of magnitude larger than that of typical "rotating spoke" phenomena. Several physical and numerical considerations are presented to more accurately understand the numerical results of Tang et al. [Phys. Plasmas 19, 073519 (2012)] in light of previous studies. (C) 2013 American Institute of Physics. [http://dx.doi.org/10.1063/1.4773895] C1 [Ellison, C. L.; Parker, J. B.; Raitses, Y.; Fisch, N. J.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. [Matyash, K.] Ernst Moritz Arndt Univ Greifswald, D-17487 Greifswald, Germany. RP Ellison, CL (reprint author), Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA. OI Parker, Jeffrey/0000-0002-9079-9930 NR 17 TC 1 Z9 1 U1 2 U2 10 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 1070-664X J9 PHYS PLASMAS JI Phys. Plasmas PD JAN PY 2013 VL 20 IS 1 AR 014701 DI 10.1063/1.4773895 PG 2 WC Physics, Fluids & Plasmas SC Physics GA 122AC UT WOS:000317286200098 ER PT J AU Hatch, DR Pueschel, MJ Jenko, F Nevins, WM Terry, PW Doerk, H AF Hatch, D. R. Pueschel, M. J. Jenko, F. Nevins, W. M. Terry, P. W. Doerk, H. TI Magnetic stochasticity and transport due to nonlinearly excited subdominant microtearing modes SO PHYSICS OF PLASMAS LA English DT Article ID ELECTROMAGNETIC GYROKINETIC SIMULATIONS; GRADIENT-DRIVEN TURBULENCE; PLASMA TURBULENCE; TEARING MODES; TOKAMAK; MICROTURBULENCE; COLLISIONLESS; ELECTRONS; PHYSICS; CODE AB Subdominant, linearly stable microtearing modes are identified as the main mechanism for the development of magnetic stochasticity and transport in gyrokinetic simulations of electromagnetic ion temperature gradient driven plasma microturbulence. The linear eigenmode spectrum is examined in order to identify and characterize modes with tearing parity. Connections are demonstrated between microtearing modes and the nonlinear fluctuations that are responsible for the magnetic stochasticity and electromagnetic transport, and nonlinear coupling with zonal modes is identified as the salient nonlinear excitation mechanism. A simple model is presented, which relates the electromagnetic transport to the electrostatic transport. These results may provide a paradigm for the mechanisms responsible for electromagnetic stochasticity and transport, which can be examined in a broader range of scenarios and parameter regimes. (C) 2013 American Institute of Physics. [http://dx.doi.org/10.1063/1.4789448] C1 [Hatch, D. R.; Jenko, F.; Doerk, H.] EURATOM, Max Planck Inst Plasmaphys, D-85748 Garching, Germany. [Pueschel, M. J.; Terry, P. W.] Univ Wisconsin, Madison, WI 53706 USA. [Nevins, W. M.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Hatch, DR (reprint author), EURATOM, Max Planck Inst Plasmaphys, D-85748 Garching, Germany. FU Office of Science of the U.S. Department of Energy [DE-AC05-00OR22725]; European Research Council under the European Union [277870] FX This work was carried out using the HELIOS supercomputer system at the International Fusion Energy Research Centre, Aomori, Japan, under the Broader Approach collaboration between Euratom and Japan, implemented by Fusion for Energy and JAEA. Resources were also used at the Oak Ridge Leadership Computing Facility at the Oak Ridge National Laboratory, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC05-00OR22725. Funding was received from the European Research Council under the European Union's Seventh Framework Programme (FP7/2007-2013)/ERC Grant Agreement No. 277870. The authors wish to acknowledge useful conversations with E. Wang and W. Dorland. NR 54 TC 19 Z9 20 U1 1 U2 10 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD JAN PY 2013 VL 20 IS 1 AR 012307 DI 10.1063/1.4789448 PG 12 WC Physics, Fluids & Plasmas SC Physics GA 122AC UT WOS:000317286200035 ER PT J AU Jenkins, TG Austin, TM Smithe, DN Loverich, J Hakim, AH AF Jenkins, Thomas G. Austin, Travis M. Smithe, David N. Loverich, John Hakim, Ammar H. TI Time-domain simulation of nonlinear radiofrequency phenomena SO PHYSICS OF PLASMAS LA English DT Article ID ION-CYCLOTRON FREQUENCY; PARAMETRIC-INSTABILITIES; EDGE PLASMA; PARTICLE SIMULATIONS; BERNSTEIN WAVES; TOKAMAK PLASMAS; HYBRID; DECAY; RANGE; EXCITATION AB Nonlinear effects associated with the physics of radiofrequency wave propagation through a plasma are investigated numerically in the time domain, using both fluid and particle-in-cell (PIC) methods. We find favorable comparisons between parametric decay instability scenarios observed on the Alcator C-MOD experiment [J. C. Rost, M. Porkolab, and R. L. Boivin, Phys. Plasmas 9, 1262 (2002)] and PIC models. The capability of fluid models to capture important nonlinear effects characteristic of wave-plasma interaction (frequency doubling, cyclotron resonant absorption) is also demonstrated. (C) 2013 American Institute of Physics. [http://dx.doi.org/10.1063/1.4776704] C1 [Jenkins, Thomas G.; Austin, Travis M.; Smithe, David N.; Loverich, John] Tech X Corp, Boulder, CO 80303 USA. [Hakim, Ammar H.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. RP Jenkins, TG (reprint author), Tech X Corp, 5621 Arapahoe Ave, Boulder, CO 80303 USA. FU U.S. Department of Energy's SBIR program under a Phase I grant [DE-SC0006242] FX We are indebted to members of the RF SciDAC project for useful discussion and feedback and for suggesting the use of J. C. Rost's C-Mod data as a suitable benchmark for the PIC approach. Dr. Rost's assistance in providing figures and data is particularly appreciated. We also acknowledge the constructive comments provided by the reviewer. This research was financially supported by the U.S. Department of Energy's SBIR program under a Phase I grant, Contract DE-SC0006242. NR 43 TC 16 Z9 16 U1 0 U2 15 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 1070-664X J9 PHYS PLASMAS JI Phys. Plasmas PD JAN PY 2013 VL 20 IS 1 AR 012116 DI 10.1063/1.4776704 PG 9 WC Physics, Fluids & Plasmas SC Physics GA 122AC UT WOS:000317286200018 ER PT J AU Karimabadi, H Roytershteyn, V Wan, M Matthaeus, WH Daughton, W Wu, P Shay, M Loring, B Borovsky, J Leonardis, E Chapman, SC Nakamura, TKM AF Karimabadi, H. Roytershteyn, V. Wan, M. Matthaeus, W. H. Daughton, W. Wu, P. Shay, M. Loring, B. Borovsky, J. Leonardis, E. Chapman, S. C. Nakamura, T. K. M. TI Coherent structures, intermittent turbulence, and dissipation in high-temperature plasmas SO PHYSICS OF PLASMAS LA English DT Article ID KELVIN-HELMHOLTZ INSTABILITY; SOLAR-WIND TURBULENCE; MAGNETOHYDRODYNAMIC TURBULENCE; RECONNECTION; TRANSPORT; FIELDS; FLUID; POWER AB An unsolved problem in plasma turbulence is how energy is dissipated at small scales. Particle collisions are too infrequent in hot plasmas to provide the necessary dissipation. Simulations either treat the fluid scales and impose an ad hoc form of dissipation (e. g., resistivity) or consider dissipation arising from resonant damping of small amplitude disturbances where damping rates are found to be comparable to that predicted from linear theory. Here, we report kinetic simulations that span the macroscopic fluid scales down to the motion of electrons. We find that turbulent cascade leads to generation of coherent structures in the form of current sheets that steepen to electron scales, triggering strong localized heating of the plasma. The dominant heating mechanism is due to parallel electric fields associated with the current sheets, leading to anisotropic electron and ion distributions which can be measured with NASA's upcoming Magnetospheric Multiscale mission. The motion of coherent structures also generates waves that are emitted into the ambient plasma in form of highly oblique compressional and shear Alfven modes. In 3D, modes propagating at other angles can also be generated. This indicates that intermittent plasma turbulence will in general consist of both coherent structures and waves. However, the current sheet heating is found to be locally several orders of magnitude more efficient than wave damping and is sufficient to explain the observed heating rates in the solar wind. (C) 2013 American Institute of Physics. [http://dx.doi.org/10.1063/1.4773205] C1 [Karimabadi, H.; Roytershteyn, V.] Univ Calif San Diego, Dept Elect & Comp Engn, La Jolla, CA 92093 USA. [Wan, M.; Matthaeus, W. H.; Wu, P.; Shay, M.] Univ Delaware, Dept Phys & Astron, Newark, DE 19716 USA. [Daughton, W.; Nakamura, T. K. M.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Loring, B.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Borovsky, J.] Space Sci Inst, Boulder, CO 80301 USA. [Leonardis, E.; Chapman, S. C.] Univ Warwick, Ctr Fus Space & Astrophys, Coventry CV4 7AL, W Midlands, England. [Chapman, S. C.] Univ Tromso, Dept Math & Stat, Tomso, Norway. RP Karimabadi, H (reprint author), Univ Calif San Diego, Dept Elect & Comp Engn, La Jolla, CA 92093 USA. RI Shay, Michael/G-5476-2013; Chapman, Sandra/C-2216-2008; Daughton, William/L-9661-2013; Wan, Minping/A-1344-2011; NASA MMS, Science Team/J-5393-2013; OI Chapman, Sandra/0000-0003-0053-1584; NASA MMS, Science Team/0000-0002-9504-5214; Roytershteyn, Vadim/0000-0003-1745-7587 FU NASA [NNH11CC65C, NNX11AJ44G]; NSF [EAGER 1105084, AGS-1063439, SHINE AGS-1156094]; UK EPSRC; STFC; DOE [DE-AC05-00OR22725]; [DE-SC0004662] FX This work was partially supported by DE-SC0004662, NASA through the Heliophysics Theory Program and NNH11CC65C, and NSF through EAGER 1105084. The Delaware group (W.H.M., M.W., P.W., and M.S.) is supported by NASA (Heliophysics Theory NNX11AJ44G, Solar Probe Plus and MMS Theory programs) and by NSF (AGS-1063439 and SHINE AGS-1156094). S.C.C. acknowledges support from the UK EPSRC and STFC. Simulations were performed on Kraken provided by the NSF at NICS, on Pleiades provided by NASA's HEC Program, and resources of the National Center for Computational Sciences at Oak Ridge National Laboratory (Jaguar/Lens), which is supported by DOE under Contract No. DE-AC05-00OR22725. Visualization and analysis were performed on Nautilus and Longhorn systems using ParaView and visualization software developed by the NICS RDAV group. We acknowledge useful conversations with J. TenBarge on kinetic Alfven turbulence. We also thank the referee for useful comments that led to improvements in the paper. NR 50 TC 106 Z9 106 U1 2 U2 32 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 1070-664X J9 PHYS PLASMAS JI Phys. Plasmas PD JAN PY 2013 VL 20 IS 1 AR 012303 DI 10.1063/1.4773205 PG 15 WC Physics, Fluids & Plasmas SC Physics GA 122AC UT WOS:000317286200031 ER PT J AU Niemann, C Gekelman, W Constantin, CG Everson, ET Schaeffer, DB Clark, SE Winske, D Zylstra, AB Pribyl, P Tripathi, SKP Larson, D Glenzer, SH Bondarenko, AS AF Niemann, C. Gekelman, W. Constantin, C. G. Everson, E. T. Schaeffer, D. B. Clark, S. E. Winske, D. Zylstra, A. B. Pribyl, P. Tripathi, S. K. P. Larson, D. Glenzer, S. H. Bondarenko, A. S. TI Dynamics of exploding plasmas in a large magnetized plasma SO PHYSICS OF PLASMAS LA English DT Article ID ALFVEN-WAVE RADIATION; LASER-PRODUCED PLASMA; SHOCK-WAVES; FIELD; EXPANSION; DESIGN; ACCELERATION; PENETRATION; PROPAGATION; CLOUDS AB The dynamics of an exploding laser-produced plasma in a large ambient magneto-plasma was investigated with magnetic flux probes and Langmuir probes. Debris-ions expanding at super-Alfvenic velocity (up to M-A = 1.5) expel the ambient magnetic field, creating a large (>20 cm) diamagnetic cavity. We observe a field compression of up to B/B-0 = 1.5 as well as localized electron heating at the edge of the bubble. Two-dimensional hybrid simulations reproduce these measurements well and show that the majority of the ambient ions are energized by the magnetic piston and swept outside the bubble volume. Nonlinear shear-Alfven waves (delta B/B-0 > 25%) are radiated from the cavity with a coupling efficiency of 70% from magnetic energy in the bubble to the wave. (C) 2013 American Institute of Physics. [http://dx.doi.org/10.1063/1.4773911] C1 [Niemann, C.; Gekelman, W.; Constantin, C. G.; Everson, E. T.; Schaeffer, D. B.; Clark, S. E.; Zylstra, A. B.; Pribyl, P.; Tripathi, S. K. P.; Bondarenko, A. S.] Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA. [Winske, D.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Larson, D.; Glenzer, S. H.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Niemann, C (reprint author), Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA. EM cniemann@ucla.edu OI Larson, David/0000-0003-0814-8555 FU DOE/NSF [DE-FG02-06ER5406, NSF05-619]; DOE Office of Science Early Career Research Program [E-FOA-0000395]; Defense Threat Reduction Agency [HDTRA1-12-1-0024] FX This work was supported by the DOE/NSF Partnership in Basic Plasma Science under Contract Nos. DE-FG02-06ER5406 and NSF05-619, the DOE Office of Science Early Career Research Program (E-FOA-0000395), and the Defense Threat Reduction Agency under Contract No. HDTRA1-12-1-0024. The experiments were performed at the UCLA Basic Plasma Science Facility (BaPSF). We thank Z. Lucky, M. Nakamoto, and M. Drandell for technical support during the experiment, and A. Ng and the University of British Columbia for the donation of the high-energy laser system. NR 56 TC 15 Z9 15 U1 0 U2 30 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 1070-664X J9 PHYS PLASMAS JI Phys. Plasmas PD JAN PY 2013 VL 20 IS 1 AR 012108 DI 10.1063/1.4773911 PG 12 WC Physics, Fluids & Plasmas SC Physics GA 122AC UT WOS:000317286200010 ER PT J AU Yin, L Albright, BJ Rose, HA Montgomery, DS Kline, JL Kirkwood, RK Michel, P Bowers, KJ Bergen, B AF Yin, L. Albright, B. J. Rose, H. A. Montgomery, D. S. Kline, J. L. Kirkwood, R. K. Michel, P. Bowers, K. J. Bergen, B. TI Self-organized coherent bursts of stimulated Raman scattering and speckle interaction in multi-speckled laser beams SO PHYSICS OF PLASMAS LA English DT Article ID DECAY INSTABILITY; PLASMA; WAVE AB Nonlinear physics governing the kinetic behavior of stimulated Raman scattering (SRS) in multi-speckled laser beams has been identified in the trapping regime over a wide range of k lambda(D) values (here k is the wave number of the electron plasma waves and lambda(D) is the Debye length) in homogeneous and inhomogeneous plasmas. Hot electrons from intense speckles, both forward and side-loss hot electrons produced during SRS daughter electron plasma wave bowing and filamentation, seed and enhance the growth of SRS in neighboring speckles by reducing Landau damping. Trapping-enhanced speckle interaction through transport of hot electrons, backscatter, and sidescatter SRS light waves enable the system of speckles to self-organize and exhibit coherent, sub-ps SRS bursts with more than 100% instantaneous reflectivity, resulting in an SRS transverse coherence width much larger than a speckle width and a SRS spectrum that peaks outside the incident laser cone. SRS reflectivity is found to saturate above a threshold laser intensity at a level of reflectivity that depends on k lambda(D): higher k lambda(D) leads to lower SRS and the reflectivity scales as similar to(k lambda(D))(-4). As k lambda(D) and Landau damping increase, speckle interaction via sidescattered light and side-loss hot electrons decreases and the occurrence of self-organized events becomes infrequent, leading to the reduction of time-averaged SRS reflectivity. It is found that the inclusion of a moderately strong magnetic field in the laser direction can effectively control SRS by suppressing transverse speckle interaction via hot electron transport. (C) 2013 American Institute of Physics. [http://dx.doi.org/10.1063/1.4774964] C1 [Yin, L.; Albright, B. J.; Rose, H. A.; Montgomery, D. S.; Kline, J. L.; Bowers, K. J.; Bergen, B.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Kirkwood, R. K.; Michel, P.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Yin, L (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM lyin@lanl.gov RI Michel, Pierre/J-9947-2012; OI Albright, Brian/0000-0002-7789-6525; Yin, Lin/0000-0002-8978-5320; Kline, John/0000-0002-2271-9919 FU U.S. Dept. of Energy by the Los Alamos National Security, LLC Los Alamos National Laboratory; DOE NNSA; LANL Directed Research and Development (LDRD) Program; DOE Office of Fusion Energy Science FX This work was performed under the auspices of the U.S. Dept. of Energy by the Los Alamos National Security, LLC Los Alamos National Laboratory and was supported by DOE NNSA Funding for ICF, by the LANL Directed Research and Development (LDRD) Program, and by the DOE Office of Fusion Energy Science. VPIC simulations were run on ASC Roadrunner and Cielo, and on DOE OLCF Jaguar. The authors acknowledge stimulating discussions with Dr. J. C. Fernandez, Dr. J. Moody, Dr. B. Afeyan and we thank Dr. R. London especially for detailed discussion on the density variation obtained in radiation hydrodynamic modeling of recent large-scale LPI experiments using the OMEGA laser. NR 36 TC 18 Z9 18 U1 1 U2 16 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD JAN PY 2013 VL 20 IS 1 AR 012702 DI 10.1063/1.4774964 PG 13 WC Physics, Fluids & Plasmas SC Physics GA 122AC UT WOS:000317286200053 ER PT J AU Aranson, IS AF Aranson, I. S. TI Active colloids SO PHYSICS-USPEKHI LA English DT Review ID SOFT CONDENSED MATTER; GRANULAR MEDIA; PARTICLES; CRYSTALS; INTERFACE; DYNAMICS; BEHAVIOR; BANDGAP; FIELDS; ROUTE AB A colloidal suspension is a heterogeneous fluid containing solid microscopic particles. Colloids play an important role in our everyday life, from food and pharmaceutical industries to medicine and nanotechnology. It is useful to distinguish two major classes of colloidal suspensions: equilibrium and active, i.e., maintained out of thermodynamic equilibrium by external electric or magnetic fields, light, chemical reactions, or hydrodynamic shear flow. While the properties of equilibrium colloidal suspensions are fairly well understood, active colloids pose a formidable challenge, and the research is in its early exploratory stage. One of the most remarkable properties of active colloids is the possibility of dynamic self-assembly, a natural tendency of simple building blocks to organize into complex functional architectures. Examples range from tunable, self-healing colloidal crystals and membranes to self-assembled microswimmers and robots. Active colloidal suspensions may exhibit material properties not present in their equilibrium counterparts, e.g., reduced viscosity and enhanced self-diffusivity, etc. This study surveys the most recent developments in the physics of active colloids, both in synthetic and living systems, with the aim of elucidation of the fundamental physical mechanisms governing self-assembly and collective behavior. C1 [Aranson, I. S.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Aranson, I. S.] Northwestern Univ, Dept Engn Sci & Appl Math, Evanston, IL 60208 USA. RP Aranson, IS (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM aronson@anl.gov RI Aranson, Igor/I-4060-2013 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Science and Engineering [DEAC02-06CH11357] FX This work was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Science and Engineering, under Contract DEAC02-06CH11357. NR 114 TC 24 Z9 24 U1 9 U2 119 PU TURPION LTD PI BRISTOL PA C/O TURPION LTD, IOP PUBLISHING, TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6HG, ENGLAND SN 1063-7869 EI 1468-4780 J9 PHYS-USP+ JI Phys. Usp. PY 2013 VL 56 IS 1 BP 79 EP 92 DI 10.3367/UFNe.0183.201301e.0087 PG 14 WC Physics, Multidisciplinary SC Physics GA 125YS UT WOS:000317578800004 ER PT J AU Vasdekis, AE AF Vasdekis, Andreas E. TI Single microbe trap and release in sub-microfluidics SO RSC ADVANCES LA English DT Article ID ELECTRON-BEAM LITHOGRAPHY; CELL ISOLATION; RESOLUTION; BACTERIA; SU-8; MICROBIOLOGY; OPTOFLUIDICS; GROWTH; ARRAYS; RESIST AB Life on Earth is comprised mostly of microbes with significant implications in disease and carbon cycling. However, their dimensions and mobility make microbes challenging to analyse on-chip. A sub-micron resolution microfluidic system (sub-microfluidics) capable of trapping and releasing single Escherichia coli bacteria is presented. The fabrication method based on electron-beam and cast molding lithography is described, as well as the trap and release of single E. coli. The release time from the trap is found to depend on cell morphology. C1 [Vasdekis, Andreas E.] Ecole Polytech Fed Lausanne, Opt Lab, Lausanne, Switzerland. [Vasdekis, Andreas E.] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. RP Vasdekis, AE (reprint author), Ecole Polytech Fed Lausanne, Opt Lab, Lausanne, Switzerland. EM andreas.vasdekis@pnnl.gov OI Vasdekis, Andreas/0000-0003-4315-1047 NR 35 TC 6 Z9 6 U1 1 U2 40 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2046-2069 J9 RSC ADV JI RSC Adv. PY 2013 VL 3 IS 18 BP 6343 EP 6346 DI 10.1039/c3ra40369f PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA 126AT UT WOS:000317584200021 ER PT S AU Beebe-Wang, J Vaska, P Dilmanian, FA Peggs, SG Schlyer, DJ AF Beebe-Wang, Joanne Vaska, Paul Dilmanian, F. Avraham Peggs, Stephen G. Schlyer, David J. BE Belkic, D TI Verifying Radiation Treatment in Proton Therapy via PET Imaging of the Induced Positron-Emitters SO THEORY OF HEAVY ION COLLISION PHYSICS IN HADRON THERAPY SE Advances in Quantum Chemistry LA English DT Review; Book Chapter ID BEAM RANGE VERIFICATION; MONTE-CARLO CODE; DISTRIBUTIONS; RADIOTHERAPY; TRANSPORT AB Positron Emission Topography (PET) is a promising technique to verify the dose distribution from proton therapy, a precise treatment modality increasingly used in radiation oncology because its radiation pattern conforms more closely to the configuration of a tumor than does that from X-ray radiation, thereby sparing normal healthy tissue. Proton therapy produces positron-emitting isotopes along the beam's path, allowing PET to image the distribution of therapeutic energy, viz., a form of quality assurance of the treatment. This ability is especially important when treating heterogeneous organs, such as the lungs or the head-and-neck, where calculating the expected dose distribution for treatment is complex. Here, we present the findings from our Monte Carlo simulations of the yield of positron emitters produced by proton beams of up to 250 MeV, followed by our statistically realistic Monte Carlo simulation of the images expected from a clinical PET scanner. Our emphases lay in predicting accurately the distribution of positron emitters, and in determining the quality of the PET signal near the Bragg peak that is critical to the success of PET imaging for verifying the proton beam's location and dosimetry. We also demonstrate that the results depend strongly on the accuracy of the available nuclear reaction cross section data. Accordingly, we quantify the differences in the calculated positron-emitter yields from four different sets of such data, comparing them to the simulated distributions of positron-emitter production and absorbed proton energies. C1 [Beebe-Wang, Joanne; Vaska, Paul; Dilmanian, F. Avraham; Peggs, Stephen G.; Schlyer, David J.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Beebe-Wang, J (reprint author), Brookhaven Natl Lab, POB 5000, Upton, NY 11973 USA. NR 32 TC 0 Z9 0 U1 0 U2 9 PU ELSEVIER ACADEMIC PRESS INC PI SAN DIEGO PA 525 B STREET, SUITE 1900, SAN DIEGO, CA 92101-4495 USA SN 0065-3276 BN 978-0-12-396455-7 J9 ADV QUANTUM CHEM JI Adv. Quantum Chem. PY 2013 VL 65 BP 111 EP 127 DI 10.1016/B978-0-12-396455-7.00005-4 PG 17 WC Chemistry, Physical SC Chemistry GA BEL65 UT WOS:000317240800006 ER PT J AU Yoon, H Hart, DB McKenna, SA AF Yoon, Hongkyu Hart, David B. McKenna, Sean A. TI Parameter estimation and predictive uncertainty in stochastic inverse modeling of groundwater flow: Comparing null-space Monte Carlo and multiple starting point methods SO WATER RESOURCES RESEARCH LA English DT Article ID SIMULATED TRANSMISSIVITY FIELDS; STEADY-STATE FLOW; ERROR REDUCTION; PILOT POINTS; 2 STATISTICS; HYDRAULIC CONDUCTIVITY; AUTOMATED CALIBRATION; NEW-MEXICO; TRANSPORT; IDENTIFIABILITY AB Given a highly parameterized groundwater model in which the conceptual model of the heterogeneity is stochastic, a set of inverse calibrations from multiple starting points (MSPs) provide an ensemble of calibrated parameters and follow-on transport predictions. However, the multiple calibrations are computationally expensive. A recently developed null-space Monte Carlo (NSMC) method combines the calibration solution-space parameters with the ensemble of null-space parameters, creating sets of calibration-constrained parameters for input to follow-on transport predictions. The consistency between probabilistic ensembles of parameter estimates and predictions created using the MSP calibration and the NSMC approaches is examined using a highly parameterized (>1300 parameters) model of the Culebra dolomite previously developed for the Waste Isolation Pilot Plant project in New Mexico as a test case. A total of 100 estimated fields are retained from the MSP approach, and the ensemble of results defining the model fit to the data and prediction of an advective travel time are compared with the same results obtained using NSMC. We demonstrate that the NSMC fields based on a single calibrated model can be significantly constrained by the calibrated solution space, and the resulting distribution of advective travel times is biased toward the travel time from the single calibrated field. To overcome this, newly proposed strategies to employ a multiple calibration-constrained NSMC (M-NSMC) approach are evaluated. Comparison of the M-NSMC and MSP methods demonstrates that M-NSMC can provide a computationally efficient and practical solution for predictive uncertainty analysis in highly nonlinear and complex subsurface flow and transport models. Citation: Yoon, H., D. B. Hart, and S. A. McKenna (2013), Parameter estimation and predictive uncertainty in stochastic inverse modeling of groundwater flow: Comparing null-space Monte Carlo and multiple starting point methods, Water Resour. Res., 49, doi: 10.1002/wrcr.20064. C1 [Yoon, Hongkyu; Hart, David B.; McKenna, Sean A.] Sandia Natl Labs, Geosci Res & Applicat Ctr, Albuquerque, NM 87185 USA. RP Yoon, H (reprint author), Sandia Natl Labs, Geosci Res & Applicat Ctr, POB 5800,MS 0751, Albuquerque, NM 87185 USA. EM hyoon@sandia.gov FU Center for Frontiers of Subsurface Energy Security, an Energy Frontier Research Center; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001114]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This material is based upon work supported as part of the Center for Frontiers of Subsurface Energy Security, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under award DE-SC0001114. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. We also acknowledge the effort of Randall Hunt and two anonymous reviewers for their careful and constructive reviews, which led to significant improvement of our manuscript. NR 62 TC 7 Z9 7 U1 1 U2 23 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0043-1397 J9 WATER RESOUR RES JI Water Resour. Res. PD JAN PY 2013 VL 49 IS 1 BP 536 EP 553 DI 10.1002/wrcr.20064 PG 18 WC Environmental Sciences; Limnology; Water Resources SC Environmental Sciences & Ecology; Marine & Freshwater Biology; Water Resources GA 129GR UT WOS:000317827600040 ER PT J AU Jung, Y Pruess, K AF Jung, Yoojin Pruess, Karsten TI Reply to comment by Maier and Kocabas on "A closed-form analytical solution for thermal single-well injection-withdrawal tests" SO WATER RESOURCES RESEARCH LA English DT Editorial Material C1 [Jung, Yoojin; Pruess, Karsten] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Jung, Y (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. EM yoojinjung@lbl.gov RI Jung, Yoojin/G-2519-2015 NR 3 TC 1 Z9 1 U1 0 U2 7 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0043-1397 J9 WATER RESOUR RES JI Water Resour. Res. PD JAN PY 2013 VL 49 IS 1 BP 644 EP 646 DI 10.1029/2012WR012827 PG 3 WC Environmental Sciences; Limnology; Water Resources SC Environmental Sciences & Ecology; Marine & Freshwater Biology; Water Resources GA 129GR UT WOS:000317827600049 ER PT J AU Yoo, B Afzal, W Prausnitz, JM AF Yoo, Brian Afzal, Waheed Prausnitz, John M. TI Effect of Water on the Densities and Viscosities of Some Ionic Liquids Containing a Phosphonium Cation SO ZEITSCHRIFT FUR PHYSIKALISCHE CHEMIE-INTERNATIONAL JOURNAL OF RESEARCH IN PHYSICAL CHEMISTRY & CHEMICAL PHYSICS LA English DT Article DE Viscosity; Density; Water Content; Trihexyltetradecylphosphonium bis(2,4,4-trimethylpentyl)phosphinate; Trihexyltetradecylphosphonium Dicyanamide; Tributyltetradecylphosphonium Dodecylbenzenesulfonate; Triisobutylmethylphosphonium Tosylate ID TEMPERATURE AB A small amount of water can significantly decrease the viscosity of an ionic liquid. From 25-80 degrees C, densities and viscosities were measured for dilute solutions of water in six ionic liquids: trihexyltetradecylphosphonium bis(2,4,4-trimethylpentyl)phosphinate, trihexyltetradecylphosphonium dicyanamide, tributyltetradecylphosphonium dodecylbenzenesulfonate, 1-ethyl,3-methylimidazolium bis(triflouromethylsulfonyl)imide, methyltrioctylammonium bis(trifluoromethylsulfonyl)imide, and triisobutylmethylphosphonium tosylate. At 25 degrees C, when the water content is about 1 wt. %, the viscosity of a phosphonium-based ionic liquid is reduced by nearly one order of magnitude. C1 [Prausnitz, John M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. RP Prausnitz, JM (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. EM prausnit@cchem.berkeley.edu OI Afzal, Waheed/0000-0002-2927-0114 FU Environmental Energy Technologies Division, Lawrence Berkeley National Laboratory FX The authors are grateful to the Environmental Energy Technologies Division, Lawrence Berkeley National Laboratory, for financial support, to Sasisanker Padmanabhan for helpful discussions, and to Prof. Michael Manga (UC Berkeley) for providing the density meter. NR 11 TC 9 Z9 9 U1 3 U2 27 PU WALTER DE GRUYTER GMBH PI BERLIN PA GENTHINER STRASSE 13, D-10785 BERLIN, GERMANY SN 0942-9352 J9 Z PHYS CHEM JI Z. Phys. Chemie-Int. J. Res. Phys. Chem. Chem. Phys. PY 2013 VL 227 IS 2-3 SI SI BP 157 EP 165 DI 10.1524/zpch.2013.0328 PG 9 WC Chemistry, Physical SC Chemistry GA 125HI UT WOS:000317530500002 ER PT J AU Chou, SS Kaehr, B Kim, J Foley, BM De, M Hopkins, PE Huang, J Brinker, CJ Dravid, VP AF Chou, Stanley S. Kaehr, Bryan Kim, Jaemyung Foley, Brian M. De, Mrinmoy Hopkins, Patrick E. Huang, Jiaxing Brinker, C. Jeffrey Dravid, Vinayak P. TI Chemically Exfoliated MoS2 as Near-Infrared Photothermal Agents SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE dichalcogenides; molybdenum; organicinorganic hybrid composites; photothermal therapy; supramolecular chemistry ID REDUCED GRAPHENE OXIDE; SINGLE-LAYER MOS2; NANOPARTICLE RECEPTORS; ALPHA-CHYMOTRYPSIN; CARBON NANOTUBES; LARGE-AREA; HEAT-FLOW; THERAPY; BINDING; PHOTOTRANSISTORS C1 [Kaehr, Bryan; Brinker, C. Jeffrey] Sandia Natl Labs, Adv Mat Lab, Albuquerque, NM 87106 USA. [Kaehr, Bryan; Brinker, C. Jeffrey] Univ New Mexico, Dept Chem, Albuquerque, NM 87106 USA. [Kaehr, Bryan; Brinker, C. Jeffrey] Univ New Mexico, Nucl Engn Ctr Microengn Mat, Albuquerque, NM 87106 USA. [Chou, Stanley S.; Kim, Jaemyung; Foley, Brian M.; De, Mrinmoy; Huang, Jiaxing; Dravid, Vinayak P.] Northwestern Univ, Dept Mat Sci & Engn, Int Inst Nanotechnol, Evanston, IL 60208 USA. [Hopkins, Patrick E.] Univ Virginia, Dept Mech & Aerosp Engn, Charlottesville, VA 22904 USA. RP Chou, SS (reprint author), Northwestern Univ, Dept Mat Sci & Engn, Int Inst Nanotechnol, Evanston, IL 60208 USA. EM s-chou@northwestern.edu; bjkaehr@sandia.gov RI Kim, Jaemyung/E-4617-2012; Huang, Jiaxing/B-7521-2009; Dravid, Vinayak/B-6688-2009; Huang, Jiaxing/A-9417-2012; OI Kim, Jaemyung/0000-0001-6144-9766; Kim, Jaemyung/0000-0002-0195-1460 FU U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences (BES), Division of Materials Sciences and Engineering; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; D.H.S.; National Cancer Institute Center for Cancer Nanotechnology Excellence (CCNE) initiative at Northwestern University [U54A119341]; National Science Foundation [0955612]; Alfred P. Sloan Research Foundation FX B.K. and C.J.B. acknowledge support from the U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences (BES), Division of Materials Sciences and Engineering. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract number DE-AC04-94AL85000. S. C. thanks D.H.S. for a fellowship and Dr. Y. Lin for helpful discussions. V. P. D. acknowledges support by the National Cancer Institute Center for Cancer Nanotechnology Excellence (CCNE) initiative at Northwestern University award number U54A119341. J.H. acknowledges support from the National Science Foundation (DMR CAREER grant number 0955612) and the Alfred P. Sloan Research Foundation. NR 51 TC 136 Z9 137 U1 37 U2 356 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PY 2013 VL 52 IS 15 BP 4160 EP 4164 DI 10.1002/anie.201209229 PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA 118YX UT WOS:000317064600015 PM 23471666 ER PT J AU Thomas, JL Raut, JC Law, KS Marelle, L Ancellet, G Ravetta, F Fast, JD Pfister, G Emmons, LK Diskin, GS Weinheimer, A Roiger, A Schlager, H AF Thomas, J. L. Raut, J. -C. Law, K. S. Marelle, L. Ancellet, G. Ravetta, F. Fast, J. D. Pfister, G. Emmons, L. K. Diskin, G. S. Weinheimer, A. Roiger, A. Schlager, H. TI Pollution transport from North America to Greenland during summer 2008 SO ATMOSPHERIC CHEMISTRY AND PHYSICS LA English DT Article ID BIOMASS BURNING EMISSIONS; MOZAIC AIRBORNE PROGRAM; LONG-RANGE TRANSPORT; ARCTIC AIR-POLLUTION; TROPOSPHERIC OZONE; CARBON-MONOXIDE; SATELLITE-OBSERVATIONS; LOWER STRATOSPHERE; SOURCE ATTRIBUTION; BOUNDARY-LAYER AB Ozone pollution transported to the Arctic is a significant concern because of the rapid, enhanced warming in high northern latitudes, which is caused, in part, by short-lived climate forcers, such as ozone. Long-range transport of pollution contributes to background and episodic ozone levels in the Arctic. However, the extent to which plumes are photochemically active during transport, particularly during the summer, is still uncertain. In this study, regional chemical transport model simulations are used to examine photochemical production of ozone in air masses originating from boreal fire and anthropogenic emissions over North America and during their transport toward the Arctic during early July 2008. Model results are evaluated using POLARCAT aircraft data collected over boreal fire source regions in Canada (ARCTAS-B) and several days downwind over Greenland (POLARCAT-France and POLARCAT-GRACE). Model results are generally in good agreement with the observations, except for certain trace gas species over boreal fire regions, in some cases indicating that the fire emissions are too low. Anthropogenic and biomass burning pollution (BB) from North America was rapidly uplifted during transport east and north to Greenland where pollution plumes were observed in the mid-and upper troposphere during POLARCAT. A model sensitivity study shows that CO levels are in better agreement with POLARCAT measurements (fresh and aged fire plumes) upon doubling CO emissions from fires. Analysis of model results, using Delta O-3/Delta CO enhancement ratios, shows that pollution plumes formed ozone during transport towards the Arctic. Fresh anthropogenic plumes have average Delta O-3/Delta CO enhancement ratios of 0.63 increasing to 0.92 for aged anthropogenic plumes, indicating additional ozone production during aging. Fresh fire plumes are only slightly enhanced in ozone (Delta O-3/Delta CO=0.08), but form ozone downwind with Delta O-3/Delta CO of 0.49 for aged BB plumes (model-based run). We estimate that aged anthropogenic and BB pollution together made an important contribution to ozone levels with an average contribution for latitudes > 55 degrees N of up to 6.5 ppbv (18%) from anthropogenic pollution and 3 ppbv (5.2%) from fire pollution in the model domain in summer 2008. C1 [Thomas, J. L.; Raut, J. -C.; Law, K. S.; Marelle, L.; Ancellet, G.; Ravetta, F.] Univ Versailles St Quentin, UPMC Univ Paris 06, CNRS, INSU,LATMOS,IPSL,UMR8190, Paris, France. [Fast, J. D.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Pfister, G.; Emmons, L. K.; Weinheimer, A.] Natl Ctr Atmospher Res, Boulder, CO 80307 USA. [Diskin, G. S.] NASA Langley Res Ctr, Hampton, VA USA. [Roiger, A.; Schlager, H.] Deutsch Zentrum Luft & Raumfahrt DLR, Inst Phys Atmosphare, Oberpfaffenhofen, Germany. RP Thomas, JL (reprint author), Univ Versailles St Quentin, UPMC Univ Paris 06, CNRS, INSU,LATMOS,IPSL,UMR8190, Paris, France. EM jennie.thomas@latmos.ipsl.fr RI Raut, Jean-Christophe/G-3946-2016; Emmons, Louisa/R-8922-2016; OI Emmons, Louisa/0000-0003-2325-6212; Raut, Jean-Christophe/0000-0002-3552-2437 FU French Agence Nationale de la Recherche (ANR); CNES; CNRS-INSU-LEFE; IPEV; EUFAR; ANR Climate Impact of Short-lived Climate Forcers and Methane in the Arctic (CLIMSLIP) Blanc SIMI [5-6 021 01]; CLIMSLIP-LEFE (CNRS-INSU); European Union Arctic Climate Change, Economy and Society (ACCESS) project [FP7-SCP0-2011-265863]; US Department of Energy (DOE) Office of Science (BER) Climate Change Modeling Program; INSU-CNRS (France); Meteo-France; Forschungszentrum (FZJ, Julich, Germany); National Science Foundation FX We thank the POLARCAT aircraft teams especially the NASA ARCTAS, DLR-GRACE, and French ATR-42 teams. French ATR-42 campaigns and data analysis were part of POLARCAT-France funded by French Agence Nationale de la Recherche (ANR), CNES, CNRS-INSU-LEFE, IPEV and EUFAR. Authors (J. Thomas, K. Law and J. C. Raut) acknowledge support from projects ANR Climate Impact of Short-lived Climate Forcers and Methane in the Arctic (CLIMSLIP) Blanc SIMI 5-6 021 01, CLIMSLIP-LEFE (CNRS-INSU), and the European Union Arctic Climate Change, Economy and Society (ACCESS) project (FP7-SCP0-2011-265863). J. Fast was supported by the US Department of Energy (DOE) Office of Science (BER) Climate Change Modeling Program. We thank D. Blake and E. Apel (NMHC measurements) as well as Greg Huey (PAN measurements) and the entire ARCTAS team for the use of the measurements taken onboard the DC8. The authors acknowledge the strong support of the European Commission, Airbus, and the Airlines (Lufthansa, Austrian, Air France) who carry free of charge the MOZAIC equipment and perform the maintenance since 1994. MOZAIC is presently funded by INSU-CNRS (France), Meteo-France, and Forschungszentrum (FZJ, Julich, Germany). The MOZAIC database is supported by ETHER (CNES and INSU-CNRS). We also acknowledge valuable help from colleagues at PNNL, NCAR (C. Wiedinmyer, S. Walters) and LATMOS/IPSL (D. Cugnet and T. Onishi). The National Center for Atmospheric Research is operated by the University Corporation for Atmospheric Research with funding from the National Science Foundation. CNRS is acknowledged for publication cost support. NR 84 TC 14 Z9 14 U1 2 U2 26 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1680-7316 EI 1680-7324 J9 ATMOS CHEM PHYS JI Atmos. Chem. Phys. PY 2013 VL 13 IS 7 BP 3825 EP 3848 DI 10.5194/acp-13-3825-2013 PG 24 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 126HV UT WOS:000317605400020 ER PT J AU Neville, SM Halder, GJ Murray, KS Moubaraki, B Kepert, CJ AF Neville, Suzanne M. Halder, Gregory J. Murray, Keith S. Moubaraki, Boujemaa Kepert, Cameron J. TI A Family of Three-Dimensional Molecular Framework Materials Containing the Three-Connecting Ligands 2,4,6-Tris(n '-pyridyl)-1,3,5-triazine: 3-tpt and 4-tpt SO AUSTRALIAN JOURNAL OF CHEMISTRY LA English DT Article ID METAL-ORGANIC FRAMEWORKS; SPIN-CROSSOVER BEHAVIOR; POROUS MATERIALS; BUILDING-BLOCKS; DESIGN; TRANSITION; CHEMISTRY; NETWORKS; NETS; TPT=2,4,6-TRI(4-PYRIDYL)-1,3,5-TRIAZINE AB Three-dimensional (3D) framework materials containing the ligands 2,4,6-tris(4'-pyridyl)-1,3,5-triazine (4-tpt) and 2,4,6-tris(3'-pyridyl)-1,3,5-triazine (3-tpt) have been prepared and their structure and magnetic properties investigated. The [M-II(NCS)(2)(py)(4)] (M-II = Fe, Co, py = 3-tpt, and 4-tpt) coordination environments in these materials have been targeted in an effort to prepare high-dimensional coordination polymers which contain spin crossover (SCO) centres. Using Fe-II, two isotopological cubic 3D materials [Fe(NCS)(2)(4-tpt)(4/3)]center dot n(BzOH, ac) (1a(Bz, ac)) and [Fe(NCS)(2)(3-tpt)(4/3)]center dot n(BzOH, ac) (1b(Bz, ac)) were formed. However, with Co II a different 3D framework topology results, [Co(NCS)(2)(3-tpt)(4/3)]center dot(BzOH, ac) (2(Bz, ac)). Further synthetic variation leads to the isostructural 3D materials trans-[M-II(NCS)(2)(4-tpt)(4/3)]cis-[M-II(NCS)(2)(4-tpt)(2)]center dot n(tce, EtOH) (Fe: 3a(Tce, Et) and Co: 3b(Tce, Et)) which form 3D networks outside Wellsian classification - and for which uniquely both two-and three-connecting modes of 4-tpt are present in the one complex. Despite having the metal coordination environments for which SCO has previously been observed, magnetic susceptibilities of this family of materials reveal a high spin nature. C1 [Neville, Suzanne M.; Murray, Keith S.; Moubaraki, Boujemaa] Monash Univ, Sch Chem, Clayton, Vic 3800, Australia. [Halder, Gregory J.] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. [Kepert, Cameron J.] Univ Sydney, Sch Chem, Sydney, NSW 2006, Australia. RP Kepert, CJ (reprint author), Univ Sydney, Sch Chem, Sydney, NSW 2006, Australia. EM c.kepert@chem.usyd.edu.au RI Halder, Gregory/C-5357-2013; Murray, Keith/B-9518-2014; neville, suzanne/B-2254-2016; OI Kepert, Cameron/0000-0002-6105-9706 FU ARC Discovery Grant; Australian Synchrotron Research Program; Commonwealth of Australia under the Major National Research Facilities Program; National Science Foundation/Department of Energy [HE9522232, CHE0087817]; Illinois board of higher education; USA Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work was supported by an ARC Discovery Grant. The authors thank K. W. Chapman and P. Turner for their assistance collecting the synchrotron single crystal data. Use of the ChemMatCARS Sector 15 at the Advanced Photon Source was supported by the Australian Synchrotron Research Program, which was funded by the Commonwealth of Australia under the Major National Research Facilities Program. ChemMatCARS Sector 15 is also supported by the National Science Foundation/Department of Energy under grant numbers HE9522232 and CHE0087817, and by the Illinois board of higher education. Use of the Advanced Photon Source was supported by the USA Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 46 TC 5 Z9 5 U1 2 U2 37 PU CSIRO PUBLISHING PI COLLINGWOOD PA 150 OXFORD ST, PO BOX 1139, COLLINGWOOD, VICTORIA 3066, AUSTRALIA SN 0004-9425 J9 AUST J CHEM JI Aust. J. Chem. PY 2013 VL 66 IS 4 BP 452 EP 463 DI 10.1071/CH12444 PG 12 WC Chemistry, Multidisciplinary SC Chemistry GA 124YG UT WOS:000317504400008 ER PT S AU Starrfield, S Timmes, FX Hix, WR Iliadis, C Arnett, WD Meakin, C Sparks, WM AF Starrfield, S. Timmes, F. X. Hix, W. R. Iliadis, C. Arnett, W. D. Meakin, C. Sparks, W. M. BE Di Stefano, R Orio, M Moe, M TI y Hydrodynamic Studies of the Evolution of Recurrent Novae to Supernova Ia Explosions SO BINARY PATHS TO TYPE IA SUPERNOVAE EXPLOSIONS SE IAU Symposium Proceedings Series LA English DT Proceedings Paper CT 281st Symposium of the International-Astronomical-Union CY JUL 04-08, 2011 CL Padova, ITALY SP INAF, City Padova, Univ Padova, Dept Astronomy, INAF Padova Observ, ANEMOS DE stars: white dwarfs; close binaries; dwarf novae; interiors; novae; cataclysmic variables; supernovae ID ACCRETING WHITE-DWARFS; HYDROGEN SHELL FLASHES; MODELS AB We have begun new studies of the evolution of thermonuclear runaways (TNRs) in the accreted envelopes of white dwarfs (WDs). Here we focus on the recent outbursts of RS Oph (2006), U Sco (2010) and T Pyx (2011). 11 Sco explodes about every 10 years and the ejected material from the WD is helium rich. It has a short orbital period for recurrent novae (RNe) but the secondary is likely to be evolved. The WD is thought to be close in mass to the Chandrasekhar limit. T Pyx has just suffered its first outburst since 1966 and it was predicted to never experience another outburst. It has a short orbital period and has formed dust in the ejecta as this paper was being written. One important question is the secular evolution of the WD. Do the repeated outbursts cause the WD to gain or lose mass? If it is gaining mass, it could eventually reach the Chandrasekhar limit and become a Type Ia supernova (SNe Ia) if it can hide the hydrogen and helium in the system. Here, we report on our latest studies of TNRs in accreted envelopes on WDs using a variety of initial WD masses, luminosities, and mass accretion rates. Of great importance to our conclusions, we assume a solar composition (Lodders abundance distribution). We use our 1-D hydro code, NOVA, that includes the Hix and Thielemann nuclear reaction network, the Iliadis reaction rate library, the Timmes equation of state, OPAL opacities, and the new convection of Arnett, Meakin, and Young. We report on the amount of ejected mass, evolution time to explode, and whether or not the WD is growing or losing mass. C1 [Starrfield, S.; Timmes, F. X.] Arizona State Univ, Sch Earth & Space Explorat, Tempe, AZ 85287 USA. [Hix, W. R.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Iliadis, C.] Univ N Carolina, Dept Phys & Astron, Chapel Hill, NC 27599 USA. [Arnett, W. D.] Univ Arizona, Dept Astron, Tucson, AZ 85721 USA. [Meakin, C.; Sparks, W. M.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Starrfield, S (reprint author), Arizona State Univ, Sch Earth & Space Explorat, Tempe, AZ 85287 USA. EM starrfield@asu.edu; fxt44@mac.com; raph@utk.edu; iliadis@unc.edu; darnett@as.arizona.edu; casey.meakin@gmail.com; warrensparks@comcast.net RI Hix, William/E-7896-2011 OI Hix, William/0000-0002-9481-9126 NR 15 TC 0 Z9 0 U1 0 U2 2 PU CAMBRIDGE UNIV PRESS PI CAMBRIDGE PA THE PITT BUILDING, TRUMPINGTON ST, CAMBRIDGE CB2 1RP, CAMBS, ENGLAND SN 1743-9213 BN 978-1-107-01981-2 J9 IAU SYMP P SERIES JI IAU Symposium Proc. Series PY 2013 VL 281 BP 166 EP + DI 10.1017/S1743921312014937 PG 2 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA BEI40 UT WOS:000316706100039 ER PT S AU Scannapieco, E Raskin, C Della Valle, M Fryer, C Rhoads, J Rockefeller, G Timmes, FX AF Scannapieco, E. Raskin, C. Della Valle, M. Fryer, C. Rhoads, J. Rockefeller, G. Timmes, F. X. BE Di Stefano, R Orio, M Moe, M TI Constraining Type Ia Supernova Progenitors SO BINARY PATHS TO TYPE IA SUPERNOVAE EXPLOSIONS SE IAU Symposium Proceedings Series LA English DT Proceedings Paper CT 281st Symposium of the International-Astronomical-Union CY JUL 04-08, 2011 CL Padova, ITALY SP INAF, City Padova, Univ Padova, Dept Astronomy, INAF Padova Observ, ANEMOS DE supernovae ID GAMMA-RAY BURSTS; CORE-COLLAPSE SUPERNOVAE; HOST GALAXIES; WHITE-DWARFS; COLLISIONS AB We present observational and theoretical studies constraining Type Ia supernova progenitors. First, we use a new observational technique to show that "prompt" SNe Ia that trace star-formation on cosmic timescales exhibit a significant delay time of 200-500 million years. This implies that either the majority of SNe Ia companion stars have main-sequence masses less than three solar masses, or that most SNe Ia arise from double-white dwarf binaries. Second we present a comprehensive study of white dwarf collisions as an avenue for creating SNe Ia. Using a smooth particle hydrodynamics code with a 13-isotope nuclear network, we show that several combinations of white dwarf masses and impact parameters produce enough Ni-56 to result in luminosities ranging from those of sub-luminous to super-luminous SNe Ia, depending on the parameters of the collision. Finally, we conduct a simulation survey of double-degenerate white dwarf mergers with varying mass combinations. Unlike previous works, we do not add detonations by hand to our simulations, and we do not find any thermonuclear explosions during the mergers. Instead, all but one of our simulations forms a cold, degenerate core surrounded by a hot disk, while our least massive pair of stars forms only a hot disk. We characterize the remnants by core mass, rotational velocity, and half-mass radius, and discuss how we will evolve them further with simulations that incorporate dissipative processes. Such simulations may indeed lead to double-degenerate Type Ia explosions that occur many orbits after the mergers themselves. C1 [Scannapieco, E.; Raskin, C.; Rhoads, J.; Timmes, F. X.] Arizona State Univ, Sch Earth & Space Explorat, Tempe, AZ 85287 USA. [Della Valle, M.] Osserv Astron Capodimonte, INAF, I-1680131 Naples, Italy. [Rhoads, J.; Rockefeller, G.] Los Alamos Natl Lab, CCS 2, Los Alamos, NM USA. RP Scannapieco, E (reprint author), Arizona State Univ, Sch Earth & Space Explorat, Tempe, AZ 85287 USA. EM evan.scannapieco@asu.edu; dellavalle@na.astro.it OI Rockefeller, Gabriel/0000-0002-9029-5097 FU NSF [AST08-06720]; NASA NESSF [PVSO401] FX This work was supported by NSF grant AST08-06720 and NASA NESSF grant PVSO401. NR 19 TC 0 Z9 0 U1 0 U2 0 PU CAMBRIDGE UNIV PRESS PI CAMBRIDGE PA THE PITT BUILDING, TRUMPINGTON ST, CAMBRIDGE CB2 1RP, CAMBS, ENGLAND SN 1743-9213 BN 978-1-107-01981-2 J9 IAU SYMP P SERIES JI IAU Symposium Proc. Series PY 2013 VL 281 BP 275 EP + DI 10.1017/S1743921312015190 PG 3 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA BEI40 UT WOS:000316706100065 ER PT J AU Berryman, E Marshall, JD Rahn, T Litvak, M Butnor, J AF Berryman, E. Marshall, J. D. Rahn, T. Litvak, M. Butnor, J. TI Decreased carbon limitation of litter respiration in a mortality-affected pinon-juniper woodland SO BIOGEOSCIENCES LA English DT Article ID PONDEROSA PINE FORESTS; SOIL RESPIRATION; PRECIPITATION PULSES; DESERT ECOSYSTEM; NITROGEN AVAILABILITY; PLANT; DECOMPOSITION; TEMPERATURE; RESPONSES; MOISTURE AB Microbial respiration depends on microclimatic variables and carbon (C) substrate availability, all of which are altered when ecosystems experience major disturbance. Widespread tree mortality, currently affecting pinon-juniper ecosystems in southwestern North America, may affect C substrate availability in several ways, for example, via litterfall pulses and loss of root exudation. To determine pinon mortality effects on C and water limitation of microbial respiration, we applied field amendments (sucrose and water) to two pinon-juniper sites in central New Mexico, USA: one with a recent (<1 yr), experimentally induced mortality event and a nearby site with live canopy. We monitored the respiration response to water and sucrose applications to the litter surface and to the underlying mineral soil surface, testing the following hypotheses: (1) soil respiration in a pinon-juniper woodland is water-and labile C-limited in both the litter layer and mineral soil; (2) pinon mortality reduces the C limitation of litter respiration; and (3) pinon mortality enhances the C limitation of mineral soil respiration. Litter respiration at both sites responded to increased water availability, yet surprisingly, mineral soil respiration was not limited by water. Consistent with hypothesis 2, C limitation of litter respiration was lower at the recent mortality site compared to the intact canopy site. Applications to the mineral soil showed evidence of reduction in CO2 flux on the girdled site and a non-significant increase on the control. We speculate that the reduction may have been driven by water-induced carbonate dissolution, which serves as a sink for CO2 and would reduce the net flux. Widespread pinon mortality may decrease labile C limitation of litter respiration, at least during the first growing season following mortality. C1 [Berryman, E.] Colorado State Univ, Dept Forest & Rangeland Stewardship, Ft Collins, CO 80523 USA. [Marshall, J. D.] Univ Idaho, Dept Forest Rangeland & Fire Sci, Moscow, ID 83843 USA. [Rahn, T.] Los Alamos Natl Lab, Div Earth & Environm Sci, Los Alamos, NM 87545 USA. [Litvak, M.] Univ New Mexico, Dept Biol, Albuquerque, NM 87131 USA. [Butnor, J.] Univ Vermont, USDA, US Forest Serv, Aiken Ctr, Burlington, VT USA. RP Berryman, E (reprint author), Colorado State Univ, Dept Forest & Rangeland Stewardship, 1472 Campus Delivery, Ft Collins, CO 80523 USA. EM erin.berryman@colostate.edu RI Rahn, Thom/C-5211-2012; Butnor, John/P-9738-2016; OI Rahn, Thomas/0000-0001-8634-1348 FU Los Alamos National Laboratory's Institute for Geophysics and Planetary Physics Minigrant Program (LA-UR) [11-10329]; US Department of Energy - EPSCoR [DE-FG02-08ER46506] FX This research was supported by Los Alamos National Laboratory's Institute for Geophysics and Planetary Physics Minigrant Program (LA-UR #11-10329) and by a grant from the US Department of Energy - EPSCoR to Marcy Litvak, Thom Rahn and Bob Sinsabaugh (#DE-FG02-08ER46506). The authors would like to acknowledge the assistance of Leo Stoscheck, Daniel McInnis, and Jennifer Johnson. The authors are greatly appreciative of comments from Bob Sinsabaugh, Mike Ryan, R. Dave Evans, Jodi Johnson-Maynard, and two anonymous reviewers. NR 41 TC 8 Z9 8 U1 0 U2 40 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1726-4170 J9 BIOGEOSCIENCES JI Biogeosciences PY 2013 VL 10 IS 3 BP 1625 EP 1634 DI 10.5194/bg-10-1625-2013 PG 10 WC Ecology; Geosciences, Multidisciplinary SC Environmental Sciences & Ecology; Geology GA 118FV UT WOS:000317010600025 ER PT J AU Todd-Brown, KEO Randerson, JT Post, WM Hoffman, FM Tarnocai, C Schuur, EAG Allison, SD AF Todd-Brown, K. E. O. Randerson, J. T. Post, W. M. Hoffman, F. M. Tarnocai, C. Schuur, E. A. G. Allison, S. D. TI Causes of variation in soil carbon simulations from CMIP5 Earth system models and comparison with observations SO BIOGEOSCIENCES LA English DT Article ID GENERAL-CIRCULATION MODEL; GLOBAL VEGETATION MODEL; CLIMATE-CHANGE; TERRESTRIAL ECOSYSTEM; ORGANIC-CARBON; PERMAFROST CARBON; NET PRIMARY; TEMPERATURE SENSITIVITY; THEORETICAL-MODEL; SEASONAL CYCLE AB Stocks of soil organic carbon represent a large component of the carbon cycle that may participate in climate change feedbacks, particularly on decadal and centennial timescales. For Earth system models (ESMs), the ability to accurately represent the global distribution of existing soil carbon stocks is a prerequisite for accurately predicting future carbon-climate feedbacks. We compared soil carbon simulations from 11 model centers to empirical data from the Harmonized World Soil Database (HWSD) and the Northern Circumpolar Soil Carbon Database (NCSCD). Model estimates of global soil carbon stocks ranged from 510 to 3040 Pg C, compared to an estimate of 1260 Pg C (with a 95% confidence interval of 890-1660 Pg C) from the HWSD. Model simulations for the high northern latitudes fell between 60 and 820 Pg C, compared to 500 Pg C (with a 95% confidence interval of 380-620 Pg C) for the NCSCD and 290 PgC for the HWSD. Global soil carbon varied 5.9 fold across models in response to a 2.6-fold variation in global net primary productivity (NPP) and a 3.6-fold variation in global soil carbon turnover times. Model-data agreement was moderate at the biome level (R-2 values ranged from 0.38 to 0.97 with a mean of 0.75); however, the spatial distribution of soil carbon simulated by the ESMs at the 1 degrees scale was not well correlated with the HWSD (Pearson correlation coefficients less than 0.4 and root mean square errors from 9.4 to 20.8 kg C m(-2)). In northern latitudes where the two data sets overlapped, agreement between the HWSD and the NCSCD was poor (Pearson correlation coefficient 0.33), indicating uncertainty in empirical estimates of soil carbon. We found that a reduced complexity model dependent on NPP and soil temperature explained much of the 1 degrees spatial variation in soil carbon within most ESMs (R-2 values between 0.62 and 0.93 for 9 of 11 model centers). However, the same reduced complexity model only explained 10% of the spatial variation in HWSD soil carbon when driven by observations of NPP and temperature, implying that other drivers or processes may be more important in explaining observed soil carbon distributions. The reduced complexity model also showed that differences in simulated soil carbon across ESMs were driven by differences in simulated NPP and the parameterization of soil heterotrophic respiration (inter-model R-2 = 0.93), not by structural differences between the models. Overall, our results suggest that despite fair global-scale agreement with observational data and moderate agreement at the biome scale, most ESMs cannot reproduce grid-scale variation in soil carbon and may be missing key processes. Future work should focus on improving the simulation of driving variables for soil carbon stocks and modifying model structures to include additional processes. C1 [Todd-Brown, K. E. O.; Randerson, J. T.; Hoffman, F. M.; Allison, S. D.] Univ Calif Irvine, Dept Earth Syst Sci, Irvine, CA 92697 USA. [Post, W. M.] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. [Allison, S. D.] Univ Calif Irvine, Dept Ecol & Evolutionary Biol, Irvine, CA 92697 USA. [Tarnocai, C.] Agr & Agri Food Canada, Res Branch, Ottawa, ON K1A 0C6, Canada. [Schuur, E. A. G.] Univ Florida, Dept Biol, Gainesville, FL 32611 USA. [Hoffman, F. M.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. RP Todd-Brown, KEO (reprint author), Univ Calif Irvine, Dept Earth Syst Sci, Irvine, CA 92697 USA. EM ktoddbro@uci.edu RI Allison, Steven/E-2978-2010; Hoffman, Forrest/B-8667-2012; OI Allison, Steven/0000-0003-4629-7842; Hoffman, Forrest/0000-0001-5802-4134; Todd-Brown, Katherine/0000-0002-3109-8130 FU NSF Advancing Theory in Biology program; Decadal and Regional Climate Prediction using Earth System Models (EaSM) program [AGU-1048890]; Office of Science (BER), US Department of Energy FX We thank Shishi Lui and Yaxing Wei for assistance with the HWSD, as well as Yufang Jin for assistance with the NCSCD data set. This research was funded by grants from the NSF Advancing Theory in Biology program, the Decadal and Regional Climate Prediction using Earth System Models (EaSM; AGU-1048890) program, and the Office of Science (BER), US Department of Energy. NR 112 TC 152 Z9 153 U1 14 U2 151 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1726-4170 EI 1726-4189 J9 BIOGEOSCIENCES JI Biogeosciences PY 2013 VL 10 IS 3 BP 1717 EP 1736 DI 10.5194/bg-10-1717-2013 PG 20 WC Ecology; Geosciences, Multidisciplinary SC Environmental Sciences & Ecology; Geology GA 118FV UT WOS:000317010600032 ER PT J AU Waidmann, CR Silks, LA Wu, RL Gordon, JC AF Waidmann, Christopher R. Silks, L. A. Pete'' Wu, Ruilian Gordon, John C. TI One-pot reduction of olefin and ketone moieties by a copper-phosphine catalyst enabled by polar aprotic solvents SO CATALYSIS SCIENCE & TECHNOLOGY LA English DT Article ID ASYMMETRIC HYDROSILYLATION; CONJUGATE REDUCTION; COPPER(II)-DIPYRIDYLPHOSPHINE CATALYST; ENANTIOSELECTIVE HYDROSILYLATION; CARBONYL-COMPOUNDS; STRYKERS REAGENT; HYDRIDE; LIGANDS; COMPLEXES; MECHANISM AB One-pot reduction of both olefin and ketone moieties in a non-food biomass derived substrate using simple copper-phosphine catalysts is described. The electron rich, sterically unencumbered bis(diethylphosphino)ethane ligand used here gives an 84% yield of the product where both the olefin and ketone have been reduced in minutes using PhSiH3 and dry acetonitrile as the solvent. The coordinating ability of acetonitrile appears to be critical for effecting this one-pot reduction. Labeling experiments indicate that ketone reduction in benzene occurs predominantly via a sigma bond metathesis pathway. C1 [Waidmann, Christopher R.; Gordon, John C.] Los Alamos Natl Lab, Div Chem, Los Alamos, NM 87545 USA. [Silks, L. A. Pete''; Wu, Ruilian] Los Alamos Natl Lab, Biosci Div, Los Alamos, NM 87545 USA. RP Waidmann, CR (reprint author), Los Alamos Natl Lab, Div Chem, POB 1663, Los Alamos, NM 87545 USA. EM waidmann@lanl.gov; jgordon@lanl.gov OI Silks, Pete/0000-0002-2993-5630 FU LDRD Program at LANL FX This work was supported by the LDRD Program at LANL. NR 40 TC 1 Z9 1 U1 1 U2 20 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2044-4753 J9 CATAL SCI TECHNOL JI Catal. Sci. Technol. PY 2013 VL 3 IS 5 BP 1240 EP 1245 DI 10.1039/c3cy20762e PG 6 WC Chemistry, Physical SC Chemistry GA 126FA UT WOS:000317596800012 ER PT J AU Borfecchia, E Garino, C Salassa, L Ruiu, T Gianolio, D Zhang, XY Attenkofer, K Chen, LX Gobetto, R Sadler, PJ Lamberti, C AF Borfecchia, Elisa Garino, Claudio Salassa, Luca Ruiu, Tiziana Gianolio, Diego Zhang, Xiaoyi Attenkofer, Klaus Chen, Lin X. Gobetto, Roberto Sadler, Peter J. Lamberti, Carlo TI X-ray transient absorption structural characterization of the (MLCT)-M-3 triplet excited state of cis-[Ru(bpy)(2)(py)(2)](2+) SO DALTON TRANSACTIONS LA English DT Article ID MOLECULAR-STRUCTURES; FINE-STRUCTURE; MLCT STATE; SPECTROSCOPY; COMPLEXES; METALLOPORPHYRIN; PHOTOCHEMISTRY; STABILIZATION; SNAPSHOTS; DYNAMICS AB The excited state dynamics and structure of the photochemically active complex cis-[Ru(bpy)(2)(py)(2)](2+) have been investigated using optical transient absorption (OTA) and X-ray transient absorption (XTA) spectroscopy, and density functional theory (DFT). Upon light-excitation in aqueous solution cis-[ Ru( bpy)(2)(py)(2)](2+) undergoes ultrafast dissociation of one pyridine ligand to form cis-[Ru(bpy)(2)(py)(H2O)](2+). OTA measurements highlighted the presence of two major time components of 1700 ps and 130 ps through which the system decays to the ground-state and evolves towards the photoproduct. XTA data were acquired after 150 ps, 500 ps, and 3000 ps from laser excitation (lambda(exc) = 351 nm) and provided the transient structure of the (MLCT)-M-3 state corresponding to the longer time component in the OTA experiment. In excellent agreement with DFT, XTA shows that the (MLCT)-M-3 geometry is characterized by an elongation of the dissociating Ru-N(py) bond and a shortening of the trans Ru-N(bpy) bond with respect to the ground state. Conversely, calculations show that the (MC)-M-3 state has a highly distorted structure with Ru-N(py) bonds between 2.77-3.05 angstrom. C1 [Borfecchia, Elisa; Garino, Claudio; Ruiu, Tiziana; Gobetto, Roberto; Lamberti, Carlo] Univ Turin, Dept Chem, NIS Ctr Excellence, I-10125 Turin, Italy. [Borfecchia, Elisa; Garino, Claudio; Ruiu, Tiziana; Gobetto, Roberto; Lamberti, Carlo] Univ Turin, INSTM Reference Ctr, I-10125 Turin, Italy. [Salassa, Luca; Sadler, Peter J.] Univ Warwick, Dept Chem, Coventry CV4 7AL, W Midlands, England. [Gianolio, Diego] Diamond Light Source Ltd, Didcot OX11 0DE, Oxon, England. [Zhang, Xiaoyi; Attenkofer, Klaus; Chen, Lin X.] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. [Zhang, Xiaoyi; Attenkofer, Klaus; Chen, Lin X.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Chen, Lin X.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. RP Salassa, L (reprint author), CIC BiomaGUNE, Paseo Miramon 182, Donostia San Sebastian 20009, Spain. EM lsalassa@cicbiomagune.es; carlo.lamberti@unito.it RI biomaGUNE, CIC/J-9136-2014; Borfecchia, Elisa/M-2568-2015; Gianolio, Diego/I-9221-2012; Lamberti, Carlo/C-5901-2013; Garino, Claudio/B-5669-2014; Salassa, Luca/M-7300-2014 OI biomaGUNE, CIC/0000-0001-7690-0660; Borfecchia, Elisa/0000-0001-8374-8329; Gianolio, Diego/0000-0002-0708-4492; Lamberti, Carlo/0000-0001-8004-2312; Garino, Claudio/0000-0002-7854-6076; Salassa, Luca/0000-0002-2112-9095 FU Marie Curie Intraeuropean Fellowship [220281 PHOTORUACD]; European Research Council (ERC) [247450]; DOE-BES [DE-AC02-06CH11357]; MICINN of Spain for the Ramon y Cajal Fellowship [RYC-2011-07787]; INSTM (Florence, Italy) FX LS was supported for this work by a Marie Curie Intraeuropean Fellowship (220281 PHOTORUACD) and by the European Research Council (ERC grant no. 247450) BIO-INCMED (PJS). Use of the APS and the CNM is supported by DOE-BES under Contract No. DE-AC02-06CH11357. LS gratefully acknowledges the MICINN of Spain for the Ramon y Cajal Fellowship RYC-2011-07787. The authors are grateful to the APS for GUP 12873 and to M. Castagna and Fratelli Castagna s.r.l. for a generous travel funding to CG and TR. EB is grateful to INSTM (Florence, Italy) for having co-founded her PhD grant. NR 52 TC 17 Z9 17 U1 3 U2 66 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1477-9226 J9 DALTON T JI Dalton Trans. PY 2013 VL 42 IS 18 BP 6564 EP 6571 DI 10.1039/c3dt32865a PG 8 WC Chemistry, Inorganic & Nuclear SC Chemistry GA 126AH UT WOS:000317583000037 PM 23474490 ER PT J AU Park, SH Choi, KB Kim, MY Lee, CS AF Park, Su Han Choi, Ki Bong Kim, Myung Yoon Lee, Chang Sik TI Experimental Investigation and Prediction of Density and Viscosity of GTL, GTL-Biodiesel, and GTL-Diesel Blends As a Function of Temperature SO ENERGY & FUELS LA English DT Article ID SYNTHESIS GAS-PRODUCTION; EMISSION CHARACTERISTICS; FUEL PROPERTIES; ENGINE; LIQUID; RME AB The purpose of this study is to experimentally investigate the densities and viscosities of gas-to-liquid (GTL)-biodiesel and GTL-diesel blends for various fuel temperatures and blending ratios. The biodiesel used in this study was derived from soybean oil, and was added to GTL from 20% to 100% by volumetric ratio. In the case of the GTL-diesel blend, diesel was added at 30% and 70% by volumetric ratio. Based on the experimental results, the empirical correlations for densities and viscosities were derived for variations in fuel temperatures and blending ratios. The densities of GTL-biodiesel and GTL-diesel blends decreased linearly with increasing fuel temperature and GTL is insensitive to temperature change compared to biodiesel and diesel. The dynamic and kinematic viscosities of GTL-biodiesel and GTL-diesel blends decreased exponentially with increasing fuel temperatures. As the fuel temperatures increased, the rate of change in viscosities for the temperature change significantly decreased. The increase of biodiesel and diesel in GTL blended fuels caused an increase in density. At a given temperature, the rates of density increase in the GTL-biodiesel and GTL-diesel blends showed similar values. The rates of density increase caused by biodiesel blending were higher than that caused by diesel blending due to the high density of biodiesel. With increased fuel temperature, the variations in viscosity from the blending of biodiesel or diesel with GTL decreased. In terms of the interdependence of density and kinematic viscosity, the density and the kinematic viscosity were positively correlated. At the same density conditions, an increase in biodiesel or diesel content in GTL blended fuels caused a decrease in the kinematic viscosity of the blended fuels. C1 [Park, Su Han; Choi, Ki Bong; Lee, Chang Sik] Hanyang Univ, Sch Mech Engn, Seoul 133791, South Korea. [Kim, Myung Yoon] Hyundai Motor Grp, Automot R&D Div, Powertrain Control Syst Team, Hwaseung Si 445706, Gyeonggi Do, South Korea. [Park, Su Han] Argonne Natl Lab, Adv Photon Source, Lemont, IL 60439 USA. RP Lee, CS (reprint author), Hanyang Univ, Sch Mech Engn, 17 Haengdang Dong, Seoul 133791, South Korea. EM cslee@hanyang.ac.kr FU Second Brain Korea 21 Project; National Research Foundation of Korea (NRF); Korea government (MEST) [2011-0025295] FX This work was supported by the Second Brain Korea 21 Project and was supported by the National Research Foundation of Korea (NRF) grant funded by the Korea government (MEST) (2011-0025295). NR 22 TC 3 Z9 3 U1 6 U2 19 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0887-0624 J9 ENERG FUEL JI Energy Fuels PD JAN PY 2013 VL 27 IS 1 BP 56 EP 65 DI 10.1021/ef301150k PG 10 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA 122OP UT WOS:000317327700007 ER PT J AU Muntean, JV Libera, JA Snyder, SW Wu, TP Cronauer, DC AF Muntean, John V. Libera, Joseph A. Snyder, Seth W. Wu, Tianpin Cronauer, Donald C. TI Quantitative Nuclear Magnetic Resonance Spectroscopy as a Tool To Evaluate Chemical Modification of Deep Hydrotreated Recycled Lube Oils SO ENERGY & FUELS LA English DT Article ID ATOMIC LAYER DEPOSITION; NMR-SPECTROSCOPY; SENSITIVITY; FRACTIONS; CATALYSTS AB The applications of H-1 and C-13 nuclear magnetic resonance (NMR) and two-dimensional H-1/C-13 NMR spectroscopy have been shown to be useful techniques for the qualitative and quantitative characterization of hydrotreated recycled lube oils. The addition of hydrogen to aromatic and alkene hydrocarbons can be quantitatively and selectively measured. The decrease of oxygen/nitrogen/sulfur species can also be inferred from the reduction of specific resonances in the NMR spectra. Treated recycled lube oil was subsequently hydrotreated with Pd catalysts deposited by either atomic layer deposition (ALD) or incipient wetness impregnation (IWI) on a SiO2/Al2O3 support. In both cases, much lower hydrogenation temperatures were required than had been observed with typical NiMo or CoMo on Al2O3. In addition, the ALD-deposited catalyst was more effective for the reduction of aromatics and heteroatom components than the IWI catalyst. The lube oil fractions were of high purity (low aromaticity and low heteroatom content) even at low reaction severity. C1 [Muntean, John V.; Libera, Joseph A.; Snyder, Seth W.; Wu, Tianpin; Cronauer, Donald C.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Cronauer, DC (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. EM dccronauer@anl.gov FU U.S. Department of Energy Office of Science Laboratory [DE-AC02-06CH11357]; Advanced Manufacturing Office), under DOE Award [YN-19-01-000, 82034] FX The submitted manuscript has been created by UChicago Argonne, LLC, Operator of Argonne National Laboratory ("Argonne"). Argonne, a U.S. Department of Energy Office of Science Laboratory, is operated under Contract DE-AC02-06CH11357. Funding for this work was provided by the U.S. Department of Energy, Office of Energy Efficiency, Industrial Technologies Program (now the Advanced Manufacturing Office), under DOE Award Number YN-19-01-000, 82034. The authors thank Joseph Renk (U.S. Department of Energy) for his guidance and support. Acknowledgements are also extended to J. T. Miller of Argonne National Laboratory and J. Franceschi, J. Condela, M. Wyant, W. Gorman, and J. Parks of the ULI/CEP team for advice, support, and oil samples used in this research. NR 25 TC 0 Z9 2 U1 1 U2 24 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0887-0624 J9 ENERG FUEL JI Energy Fuels PD JAN PY 2013 VL 27 IS 1 BP 133 EP 137 DI 10.1021/ef301490d PG 5 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA 122OP UT WOS:000317327700016 ER PT J AU Smagala, TG Christensen, E Christison, KM Mohler, RE Gjersing, E McCormick, RL AF Smagala, Thomas G. Christensen, Earl Christison, Krege M. Mohler, Rachel E. Gjersing, Erica McCormick, Robert L. TI Hydrocarbon Renewable and Synthetic Diesel Fuel Blendstocks: Composition and Properties SO ENERGY & FUELS LA English DT Article ID TRANSPORTATION FUELS; BIOMASS; CATALYSTS AB We examined the chemical composition and properties of several diesel fuels and blendstocks derived from Fischer-Tropsch (FT) synthesis, hydroisomerization of lipids, and fermentation of sugar via the terpenoid metabolic pathway. Comprehensive two-dimensional gas chromatographic analysis with nonpolar and polar columns, C-13 NMR, GC-MS, and elemental analysis were used to assess fuel chemistry. Performance properties included density, heat of combustion, cetane number, and cloud point, as well as other properties. The fuels consisted almost entirely of normal and iso-paraffins. Three samples contained residual oxygen below 0.1 mass %. All of the renewable and synthetic diesel fuels have significantly lower density than is typical for a petroleum-derived diesel fuel. As a result, they have slightly higher net heat of combustion on a mass basis (2%-3% higher), but lower heat of combustion on a volume basis (3%-7% lower). Two critical diesel performance properties, cetane number and cloud point, were correlated with iso-paraffin content and chain length. The results confirm that properties of hydroisomerized fats and oils, as well as FT diesel, can be tuned by increasing the degree of isomerization to lower cloud point which also lowers the cetane number. In spite of this trade-off between cloud point, and cetane number, the cetane numbers were still over 70 for fuels with cloud points as low as -27 degrees C. The terpenoid biofuel exhibited a cloud point below -70 degrees C and a cetane number of 58. C1 [Smagala, Thomas G.; Christison, Krege M.; Mohler, Rachel E.] Chevron Corp, Richmond, CA 94801 USA. [Christensen, Earl; Gjersing, Erica; McCormick, Robert L.] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Smagala, TG (reprint author), Chevron Corp, 100 Chevron Way, Richmond, CA 94801 USA. EM tsmagala@chevron.com RI McCormick, Robert/B-7928-2011 FU Laboratory Directed Research and Development (LDRD) Program FX Work at the National Renewable Energy Laboratory (NREL) was supported by the Laboratory Directed Research and Development (LDRD) Program. NREL is a national laboratory of the U.S. Department of Energy Office of Energy Efficiency and Renewable Energy operated by the Alliance for Sustainable Energy, LLC. Part of the low-temperature performance testing was kindly supplied by Innospec Fuel Specialties. NR 23 TC 10 Z9 10 U1 2 U2 41 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0887-0624 J9 ENERG FUEL JI Energy Fuels PD JAN PY 2013 VL 27 IS 1 BP 237 EP 246 DI 10.1021/ef3012849 PG 10 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA 122OP UT WOS:000317327700029 ER PT J AU Averyt, K Macknick, J Rogers, J Madden, N Fisher, J Meldrum, J Newmark, R AF Averyt, K. Macknick, J. Rogers, J. Madden, N. Fisher, J. Meldrum, J. Newmark, R. TI Water use for electricity in the United States: an analysis of reported and calculated water use information for 2008 SO ENVIRONMENTAL RESEARCH LETTERS LA English DT Article DE energy water nexus; electricity; freshwater demands AB Water use by the electricity sector represents a significant portion of the United States water budget (41% of total freshwater withdrawals; 3% consumed). Sustainable management of water resources necessitates an accurate accounting of all water demands, including water use for generation of electricity. Since 1985, the Department of Energy (DOE) Energy Information Administration (EIA) has collected self-reported data on water consumption and withdrawals from individual power generators. These data represent the only annual collection of water consumption and withdrawals by the electricity sector. Here, we compile publically available information into a comprehensive database and then calculate water withdrawals and consumptive use for power plants in the US. In effect, we evaluate the quality of water use data reported by EIA for the year 2008. Significant differences between reported and calculated water data are evident, yet no consistent reason for the discrepancies emerges. C1 [Averyt, K.; Meldrum, J.] Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80305 USA. [Macknick, J.; Newmark, R.] Natl Renewable Energy Lab, Strateg Energy Anal Ctr, Golden, CO 80401 USA. [Rogers, J.; Madden, N.] Union Concerned Scientists, Cambridge, MA 02139 USA. [Fisher, J.] Synapse Energy Econ, Cambridge, MA 02139 USA. RP Averyt, K (reprint author), Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80305 USA. EM kristen.averyt@colorado.edu OI Meldrum, James/0000-0001-5250-3759 FU Kresge Foundation; Wallace Research Foundation; Union of Concerned Scientists; Energy Water in a Warming World (EW3); EW3 Scientific Advisory Committee FX The authors would like to thank Rachel Wilson and Nicole Hughes for their work compiling the database, as well as Shazia Davis for her contributions to this effort. This work was supported by The Kresge Foundation, Wallace Research Foundation, and Roger and Vicki Sant. We greatly appreciate the support of the Union of Concerned Scientists, The Energy Water in a Warming World (EW3) contributors, and the EW3 Scientific Advisory Committee, particularly M Webber for helpful insights and reviews. Additional support was provided through the Western Water Assessment and the Cooperative Institute for Research in Environmental Sciences at University of Colorado Boulder. NR 11 TC 28 Z9 29 U1 5 U2 35 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-9326 J9 ENVIRON RES LETT JI Environ. Res. Lett. PD JAN-MAR PY 2013 VL 8 IS 1 AR 015001 DI 10.1088/1748-9326/8/1/015001 PG 9 WC Environmental Sciences; Meteorology & Atmospheric Sciences SC Environmental Sciences & Ecology; Meteorology & Atmospheric Sciences GA 118BV UT WOS:000316998300064 ER PT J AU Clemmer, S Rogers, J Sattler, S Macknick, J Mai, T AF Clemmer, S. Rogers, J. Sattler, S. Macknick, J. Mai, T. TI Modeling low-carbon US electricity futures to explore impacts on national and regional water use SO ENVIRONMENTAL RESEARCH LETTERS LA English DT Article DE electricity; water; climate; modeling AB The US electricity sector is currently responsible for more than 40% of both energy-related carbon dioxide emissions and total freshwater withdrawals for power plant cooling (EIA 2012a Annual Energy Outlook 2012 (Washington, DC: US Department of Energy), Kenny et al 2009 Estimated Use of Water in the United States 2005 (US Geological Survey Circular vol 1344) (Reston, VA: US Geological Survey)). Changes in the future electricity generation mix in the United States will have important implications for water use, particularly given the changing water availability arising from competing demands and climate change and variability. However, most models that are used to make long-term projections of the electricity sector do not have sufficient regional detail for analyzing water-related impacts and informing important electricity-and water-related decisions. This paper uses the National Renewable Energy Laboratory's Regional Energy Deployment System (ReEDS) to model a range of low-carbon electricity futures nationally that are used to calculate changes in national water use (a sample result, on water consumption, is included here). The model also produces detailed sub-regional electricity results through 2050 that can be linked with basin-level water modeling. The results will allow for sufficient geographic resolution and detail to be relevant from a water management perspective. C1 [Clemmer, S.; Rogers, J.; Sattler, S.] Union Concerned Scientists, Cambridge, MA 02238 USA. [Macknick, J.; Mai, T.] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Clemmer, S (reprint author), Union Concerned Scientists, Cambridge, MA 02238 USA. EM sclemmer@ucsusa.org; jrogers@ucsusa.org; ssattler@ucsusa.org; Jordan.Macknick@nrel.gov; Trieu.Mai@nrel.gov FU Kresge Foundation; Wallace Research Foundation; Roger and Vicki Sant FX We gratefully acknowledge funding for this research from The Kresge Foundation, Wallace Research Foundation, and Roger and Vicki Sant, and the research oversight provided by the EW3 Scientific Advisory Committee-Peter Frumhoff (Union of Concerned Scientists), George Hornberger (Vanderbilt University), Robert Jackson (Duke University), Robin Newmark (NREL), Jonathan Overpeck (University of Arizona), Brad Udall (University of Colorado Boulder, NOAA Western Water Assessment), and Michael Webber (University of Texas at Austin). NR 39 TC 19 Z9 19 U1 0 U2 18 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-9326 J9 ENVIRON RES LETT JI Environ. Res. Lett. PD JAN-MAR PY 2013 VL 8 IS 1 AR 015004 DI 10.1088/1748-9326/8/1/015004 PG 11 WC Environmental Sciences; Meteorology & Atmospheric Sciences SC Environmental Sciences & Ecology; Meteorology & Atmospheric Sciences GA 118BV UT WOS:000316998300067 ER PT J AU Klimont, Z Smith, SJ Cofala, J AF Klimont, Z. Smith, S. J. Cofala, J. TI The last decade of global anthropogenic sulfur dioxide: 2000-2011 emissions SO ENVIRONMENTAL RESEARCH LETTERS LA English DT Article DE sulfur dioxide; global emissions; RCP; anthropogenic ID AEROSOL OPTICAL DEPTH; AIR-QUALITY; CHINA; PROJECTIONS; SCENARIOS; GASES AB The evolution of global and regional anthropogenic SO2 emissions in the last decade has been estimated through a bottom-up calculation. After increasing until about 2006, we estimate a declining trend continuing until 2011. However, there is strong spatial variability, with North America and Europe continuing to reduce emissions, with an increasing role of Asia and international shipping. China remains a key contributor, but the introduction of stricter emission limits followed by an ambitious program of installing flue gas desulfurization on power plants resulted in a significant decline in emissions from the energy sector and stabilization of total Chinese SO2 emissions. Comparable mitigation strategies are not yet present in several other Asian countries and industrial sectors in general, while emissions from international shipping are expected to start declining soon following an international agreement to reduce the sulfur content of fuel oil. The estimated trends in global SO2 emissions are within the range of representative concentration pathway (RCP) projections and the uncertainty previously estimated for the year 2005. C1 [Klimont, Z.; Cofala, J.] Int Inst Appl Syst Anal, A-2361 Laxenburg, Austria. [Smith, S. J.] Pacific NW Natl Lab, Joint Global Change Res Inst, College Pk, MD 20740 USA. RP Klimont, Z (reprint author), Int Inst Appl Syst Anal, Schlosspl 1, A-2361 Laxenburg, Austria. EM klimont@iiasa.ac.at RI Klimont, Zbigniew/P-7641-2015 OI Klimont, Zbigniew/0000-0003-2630-198X FU ECLIPSE European Union [282688, 265148]; Office of Biological and Environmental Research of the US Department of Energy FX Z Klimont and J Cofala acknowledge the support of the ECLIPSE European Union's Seventh Framework Programme (FP7/2007-2013) under Grant Agreement no. 282688 and the FP7 PEGASOS project, under Grant Agreement 265148. S Smith's work on this paper was supported by the Office of Biological and Environmental Research of the US Department of Energy as part of the Earth System Modeling Program. The authors would like to thank Stephen Dessel for assistance with data processing and Chris Heyes and Wolfgang Schopp for gridding of emissions. NR 33 TC 98 Z9 99 U1 10 U2 102 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-9326 J9 ENVIRON RES LETT JI Environ. Res. Lett. PD JAN-MAR PY 2013 VL 8 IS 1 AR 014003 DI 10.1088/1748-9326/8/1/014003 PG 6 WC Environmental Sciences; Meteorology & Atmospheric Sciences SC Environmental Sciences & Ecology; Meteorology & Atmospheric Sciences GA 118BV UT WOS:000316998300011 ER PT J AU Le Page, Y Hurtt, G Thomson, AM Bond-Lamberty, B Patel, P Wise, M Calvin, K Kyle, P Clarke, L Edmonds, J Janetos, A AF Le Page, Y. Hurtt, G. Thomson, A. M. Bond-Lamberty, B. Patel, P. Wise, M. Calvin, K. Kyle, P. Clarke, L. Edmonds, J. Janetos, A. TI Sensitivity of climate mitigation strategies to natural disturbances SO ENVIRONMENTAL RESEARCH LETTERS LA English DT Article DE natural disturbances; climate change; integrated assessment; climate mitigation; climate policies ID FOREST PRODUCTIVITY; TROPICAL CYCLONES; CARBON BALANCE; LAND-USE; FUTURE; FIRE; CO2; STABILIZATION; ENHANCEMENT; SCENARIOS AB The present and future concentration of atmospheric carbon dioxide depends on both anthropogenic and natural sources and sinks of carbon. Most proposed climate mitigation strategies rely on a progressive transition to carbon-efficient technologies to reduce industrial emissions, substantially supported by policies to maintain or enhance the terrestrial carbon stock in forests and other ecosystems. This strategy may be challenged if terrestrial sequestration capacity is affected by future climate feedbacks, but how and to what extent is little understood. Here, we show that climate mitigation strategies are highly sensitive to future natural disturbance rates (e.g. fires, hurricanes, droughts), because of the potential effect of disturbances on the terrestrial carbon balance. Generally, altered disturbance rates affect the pace of societal and technological transitions required to achieve the mitigation target, with substantial consequences on the energy sector and the global economy. An understanding of the future dynamics and consequences of natural disturbances on terrestrial carbon balance is thus essential for developing robust climate mitigation strategies and policies. C1 [Le Page, Y.; Hurtt, G.; Thomson, A. M.; Bond-Lamberty, B.; Patel, P.; Wise, M.; Calvin, K.; Kyle, P.; Clarke, L.; Edmonds, J.; Janetos, A.] Univ Maryland, Pacific NW Natl Lab, Joint Global Change Res Inst, College Pk, MD 20740 USA. [Hurtt, G.] Univ Maryland, Dept Geog Sci, College Pk, MD 20740 USA. RP Le Page, Y (reprint author), Univ Maryland, Pacific NW Natl Lab, Joint Global Change Res Inst, College Pk, MD 20740 USA. EM Yannick.LePage@pnnl.gov RI Thomson, Allison/B-1254-2010; Bond-Lamberty, Ben/C-6058-2008; OI Bond-Lamberty, Ben/0000-0001-9525-4633; Calvin, Katherine/0000-0003-2191-4189 FU NASA Terrestrial Ecology and Inter-Disciplinary Studies programs; DOE Office of Science Integrated Assessment Program FX This study was supported by grants from the NASA Terrestrial Ecology and Inter-Disciplinary Studies programs and the DOE Office of Science Integrated Assessment Program. The Global Change Assessment Model (GCAM) is freely available as a community model (www.globalchange.umd.edu/models/gcam/). NR 40 TC 10 Z9 10 U1 3 U2 37 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-9326 J9 ENVIRON RES LETT JI Environ. Res. Lett. PD JAN-MAR PY 2013 VL 8 IS 1 AR 015018 DI 10.1088/1748-9326/8/1/015018 PG 6 WC Environmental Sciences; Meteorology & Atmospheric Sciences SC Environmental Sciences & Ecology; Meteorology & Atmospheric Sciences GA 118BV UT WOS:000316998300081 ER PT J AU Meldrum, J Nettles-Anderson, S Heath, G Macknick, J AF Meldrum, J. Nettles-Anderson, S. Heath, G. Macknick, J. TI Life cycle water use for electricity generation: a review and harmonization of literature estimates SO ENVIRONMENTAL RESEARCH LETTERS LA English DT Article DE life cycle assessment; consumption; withdrawal; power; meta-analysis ID GREENHOUSE-GAS EMISSIONS; ENERGY; POWER; BIOMASS AB This article provides consolidated estimates of water withdrawal and water consumption for the full life cycle of selected electricity generating technologies, which includes component manufacturing, fuel acquisition, processing, and transport, and power plant operation and decommissioning. Estimates were gathered through a broad search of publicly available sources, screened for quality and relevance, and harmonized for methodological differences. Published estimates vary substantially, due in part to differences in production pathways, in defined boundaries, and in performance parameters. Despite limitations to available data, we find that: water used for cooling of thermoelectric power plants dominates the life cycle water use in most cases; the coal, natural gas, and nuclear fuel cycles require substantial water per megawatt-hour in most cases; and, a substantial proportion of life cycle water use per megawatt-hour is required for the manufacturing and construction of concentrating solar, geothermal, photovoltaic, and wind power facilities. On the basis of the best available evidence for the evaluated technologies, total life cycle water use appears lowest for electricity generated by photovoltaics and wind, and highest for thermoelectric generation technologies. This report provides the foundation for conducting water use impact assessments of the power sector while also identifying gaps in data that could guide future research. C1 [Meldrum, J.] Univ Colorado, Western Water Assessment, Boulder, CO 80309 USA. [Meldrum, J.] Univ Colorado, Inst Behav Sci, Boulder, CO 80309 USA. [Nettles-Anderson, S.; Heath, G.; Macknick, J.] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Meldrum, J (reprint author), Univ Colorado, Western Water Assessment, Boulder, CO 80309 USA. EM james.meldrum@colorado.edu; garvin.heath@nrel.gov; jordan.macknick@nrel.gov OI Meldrum, James/0000-0001-5250-3759 FU US Department of Energy [DE-AC36-08-GO28308]; National Renewable Energy Laboratory FX This work was supported by the US Department of Energy under Contract No. DE-AC36-08-GO28308 with the National Renewable Energy Laboratory. We wish to thank Laura Vimmerstedt and Dan Bilello, whose comments helped to improve the manuscript. We also acknowledge the LCA Harmonization project team that developed the database of LCA publications (www.nrel.gov/harmonization), Alfred Hicks for polishing the graphics, and Judy Oberg for research assistance. NR 66 TC 49 Z9 50 U1 15 U2 70 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-9326 J9 ENVIRON RES LETT JI Environ. Res. Lett. PD JAN-MAR PY 2013 VL 8 IS 1 AR 015031 DI 10.1088/1748-9326/8/1/015031 PG 18 WC Environmental Sciences; Meteorology & Atmospheric Sciences SC Environmental Sciences & Ecology; Meteorology & Atmospheric Sciences GA 118BV UT WOS:000316998300094 ER PT J AU Shehabi, A Stokes, JR Horvath, A AF Shehabi, Arman Stokes, Jennifer R. Horvath, Arpad TI Reply to Comment on 'Energy and air emission implications of a decentralized wastewater system' SO ENVIRONMENTAL RESEARCH LETTERS LA English DT Editorial Material DE life-cycle assessment; decentralized wastewater treatment; greenhouse gases AB Complementing centralized water-related infrastructure with decentralized facilities is being considered in some communities and a life-cycle perspective is needed for informed decision making. Our 2012 study presents a framework for analyzing the environmental effects of decentralized wastewater systems. While the analysis framework could be applied to cases with a variety of sizes, we evaluated two currently operating systems in California, one decentralized and one centralized plant with a much larger capacity. The disparate scales of the two plants represent an 'off-the-grid' suburban neighborhood-scale system compared with a similarly sized neighborhood connecting to an adjacent large centralized plant. Deciding whether or not to connect expanding developments to nearby centralized plants is a realistic scenario for future growth, making the treatment plants evaluated in our study a realistic choice for comparison. C1 [Shehabi, Arman] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Stokes, Jennifer R.; Horvath, Arpad] Univ Calif Berkeley, Dept Civil & Environm Engn, Berkeley, CA 94720 USA. RP Shehabi, A (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. EM ashehabi@lbl.gov; horvath@ce.berkeley.edu NR 2 TC 0 Z9 0 U1 3 U2 12 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-9326 J9 ENVIRON RES LETT JI Environ. Res. Lett. PD JAN-MAR PY 2013 VL 8 IS 1 AR 019002 DI 10.1088/1748-9326/8/1/019002 PG 2 WC Environmental Sciences; Meteorology & Atmospheric Sciences SC Environmental Sciences & Ecology; Meteorology & Atmospheric Sciences GA 118BV UT WOS:000316998300106 ER PT J AU Warner, E Inman, D Kunstman, B Bush, B Vimmerstedt, L Peterson, S Macknick, J Zhang, YM AF Warner, Ethan Inman, Daniel Kunstman, Benjamin Bush, Brian Vimmerstedt, Laura Peterson, Steve Macknick, Jordan Zhang, Yimin TI Modeling biofuel expansion effects on land use change dynamics SO ENVIRONMENTAL RESEARCH LETTERS LA English DT Article DE system dynamics; biofuel; land use; agriculture; diet; sustainability ID GREENHOUSE-GAS EMISSIONS; ENERGY AB Increasing demand for crop-based biofuels, in addition to other human drivers of land use, induces direct and indirect land use changes (LUC). Our system dynamics tool is intended to complement existing LUC modeling approaches and to improve the understanding of global LUC drivers and dynamics by allowing examination of global LUC under diverse scenarios and varying model assumptions. We report on a small subset of such analyses. This model provides insights into the drivers and dynamic interactions of LUC (e. g., dietary choices and biofuel policy) and is not intended to assert improvement in numerical results relative to other works. Demand for food commodities are mostly met in high food and high crop-based biofuel demand scenarios, but cropland must expand substantially. Meeting roughly 25% of global transportation fuel demand by 2050 with biofuels requires >2 times the land used to meet food demands under a presumed 40% increase in per capita food demand. In comparison, the high food demand scenario requires greater pastureland for meat production, leading to larger overall expansion into forest and grassland. Our results indicate that, in all scenarios, there is a potential for supply shortfalls, and associated upward pressure on prices, of food commodities requiring higher land use intensity (e. g., beef) which biofuels could exacerbate. C1 [Warner, Ethan; Inman, Daniel; Kunstman, Benjamin; Bush, Brian; Vimmerstedt, Laura; Macknick, Jordan; Zhang, Yimin] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Peterson, Steve] Peterson Grp, Lebanon, NH USA. [Peterson, Steve] Lexidyne LLC, Colorado Springs, CO USA. [Peterson, Steve] Dartmouth Coll, Thayer Sch Engn, Hanover, NH 03755 USA. RP Warner, E (reprint author), Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. EM Ethan.Warner@nrel.gov OI Bush, Brian/0000-0003-2864-7028 FU US Department of Energy's Office of Biomass Program FX The authors wish to acknowledge the US Department of Energy's Office of Biomass Program which provided the funding for this work. The authors do not have any other potential conflicts of interest. Data sources used in the model are included in the supplemental information, and are cited in the references section. NR 33 TC 9 Z9 9 U1 3 U2 32 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-9326 J9 ENVIRON RES LETT JI Environ. Res. Lett. PD JAN-MAR PY 2013 VL 8 IS 1 AR 015003 DI 10.1088/1748-9326/8/1/015003 PG 10 WC Environmental Sciences; Meteorology & Atmospheric Sciences SC Environmental Sciences & Ecology; Meteorology & Atmospheric Sciences GA 118BV UT WOS:000316998300066 ER PT J AU Wei, M Nelson, JH Greenblatt, JB Mileva, A Johnston, J Ting, M Yang, C Jones, C McMahon, JE Kammen, DM AF Wei, Max Nelson, James H. Greenblatt, Jeffery B. Mileva, Ana Johnston, Josiah Ting, Michael Yang, Christopher Jones, Chris McMahon, James E. Kammen, Daniel M. TI Deep carbon reductions in California require electrification and integration across economic sectors SO ENVIRONMENTAL RESEARCH LETTERS LA English DT Article DE energy system modeling; renewable energy; long term energy scenarios; electricity system optimization; deep carbon reduction ID CUTS AB Meeting a greenhouse gas (GHG) reduction target of 80% below 1990 levels in the year 2050 requires detailed long-term planning due to complexity, inertia, and path dependency in the energy system. A detailed investigation of supply and demand alternatives is conducted to assess requirements for future California energy systems that can meet the 2050 GHG target. Two components are developed here that build novel analytic capacity and extend previous studies: (1) detailed bottom-up projections of energy demand across the building, industry and transportation sectors; and (2) a high-resolution variable renewable resource capacity planning model (SWITCH) that minimizes the cost of electricity while meeting GHG policy goals in the 2050 timeframe. Multiple pathways exist to a low-GHG future, all involving increased efficiency, electrification, and a dramatic shift from fossil fuels to low-GHG energy. The electricity system is found to have a diverse, cost-effective set of options that meet aggressive GHG reduction targets. This conclusion holds even with increased demand from transportation and heating, but the optimal levels of wind and solar deployment depend on the temporal characteristics of the resulting load profile. Long-term policy support is found to be a key missing element for the successful attainment of the 2050 GHG target in California. C1 [Wei, Max; Greenblatt, Jeffery B.; McMahon, James E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Energy Anal & Environm Impacts Dept, Berkeley, CA 94720 USA. [Nelson, James H.; Mileva, Ana; Johnston, Josiah; Jones, Chris; Kammen, Daniel M.] Univ Calif Berkeley, Energy & Resources Grp, Berkeley, CA 94720 USA. [Ting, Michael] Itron Inc, Oakland, CA 94607 USA. [Yang, Christopher] Univ Calif Davis, Inst Transportat Studies, Davis, CA 95616 USA. [Kammen, Daniel M.] Univ Calif Berkeley, Richard & Rhoda Goldman Sch Publ Policy, Berkeley, CA 94720 USA. RP Wei, M (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Energy Anal & Environm Impacts Dept, 1 Cyclotron Rd MS 90R-2002, Berkeley, CA 94720 USA. EM Mwei@lbl.gov; kammen@berkeley.edu RI Yang, Christopher/G-3725-2013 FU California Energy Commission FX We thank the California Energy Commission for support. This paper reflects the views of the authors and does not necessarily reflect the view of the California Energy Commission or the State of California. DMK thanks the Class of 1935 of the University of California, Berkeley, and the Karsten Family Foundation. NR 28 TC 15 Z9 15 U1 1 U2 30 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-9326 J9 ENVIRON RES LETT JI Environ. Res. Lett. PD JAN-MAR PY 2013 VL 8 IS 1 AR 014038 DI 10.1088/1748-9326/8/1/014038 PG 10 WC Environmental Sciences; Meteorology & Atmospheric Sciences SC Environmental Sciences & Ecology; Meteorology & Atmospheric Sciences GA 118BV UT WOS:000316998300046 ER PT J AU Tang, JY Riley, WJ Koven, CD Subin, ZM AF Tang, J. Y. Riley, W. J. Koven, C. D. Subin, Z. M. TI CLM4-BeTR, a generic biogeochemical transport and reaction module for CLM4: model development, evaluation, and application SO GEOSCIENTIFIC MODEL DEVELOPMENT LA English DT Article ID METHANE EMISSIONS; ORGANIC-CARBON; CO2 PRODUCTION; SOIL; CLIMATE; CYCLE; DECOMPOSITION; SIMULATION; DYNAMICS; EXCHANGE AB To improve regional and global biogeochemistry modeling and climate predictability, we have developed a generic reactive transport module for the land model CLM4 (called CLM4-BeTR (Biogeochemical Transport and Reactions)). CLM4-BeTR represents the transport, interactions, and biotic and abiotic transformations of an arbitrary number of tracers (aka chemical species) in an arbitrary number of phases (e. g., dissolved, gaseous, sorbed, aggregate). An operator splitting approach was employed and consistent boundary conditions were derived for each modeled sub-process. Aqueous tracer fluxes, associated with hydrological processes such as surface run-on and run-off, belowground drainage, and ice to liquid conversion were also computed consistently with the bulk water fluxes calculated by the soil physics module in CLM4. The transport code was evaluated and found in good agreement with several analytical test cases using a time step of 30 min. The model was then applied at the Harvard Forest site with a representation of depth-dependent belowground biogeochemistry. The results indicated that, at this site, (1) CLM4-BeTR was able to simulate soil-surface CO2 effluxes and soil CO2 profiles accurately; (2) the transient surface CO2 effluxes calculated based on the tracer transport mechanism were in general not equal to the belowground CO2 production rates with the magnitude of the difference being a function of averaging timescale and site conditions: differences were large (-20 similar to 20 %) on hourly, smaller (-5 similar to 5 %) at daily timescales, and persisted to the monthly timescales with a smaller magnitude (<4 %); (3) losses of CO2 through processes other than surface gas efflux were less than 1% of the overall soil respiration; and (4) the contributions of root respiration and heterotrophic respiration have distinct temporal signals in surface CO2 effluxes and soil CO2 concentrations. The development of CLM4-BeTR will allow detailed comparisons between ecosystem observations and predictions and insights to the modeling of terrestrial biogeochemistry. C1 [Tang, J. Y.; Riley, W. J.; Koven, C. D.; Subin, Z. M.] Lawrence Berkeley Natl Lab LBL, Div Earth Sci, Dept Climate & Carbon Sci, Berkeley, CA 94720 USA. RP Tang, JY (reprint author), Lawrence Berkeley Natl Lab LBL, Div Earth Sci, Dept Climate & Carbon Sci, Berkeley, CA 94720 USA. EM jinyuntang@lbl.gov RI Tang, Jinyun/M-4922-2013; Subin, Zachary/K-5168-2012; Riley, William/D-3345-2015; Koven, Charles/N-8888-2014 OI Tang, Jinyun/0000-0002-4792-1259; Subin, Zachary/0000-0002-9257-9288; Riley, William/0000-0002-4615-2304; Koven, Charles/0000-0002-3367-0065 FU Office of Science, Office of Biological and Environmental Research of the US Department of Energy [DE-AC02-05CH11231] FX This research was supported by the Director, Office of Science, Office of Biological and Environmental Research of the US Department of Energy under Contract No. DE-AC02-05CH11231 as part of their Regional and Global Climate Modeling Program. The authors appreciate Kathleen Savage and Eric Davidson at the Woods Hole Research Center for providing the soil CO2 profile data and soil moisture and temperature data at the Harvard Forest site. NR 55 TC 19 Z9 19 U1 1 U2 22 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1991-959X EI 1991-9603 J9 GEOSCI MODEL DEV JI Geosci. Model Dev. PY 2013 VL 6 IS 1 BP 127 EP 140 DI 10.5194/gmd-6-127-2013 PG 14 WC Geosciences, Multidisciplinary SC Geology GA 118FI UT WOS:000317008500009 ER PT J AU Lamarque, JF Shindell, DT Josse, B Young, PJ Cionni, I Eyring, V Bergmann, D Cameron-Smith, P Collins, WJ Doherty, R Dalsoren, S Faluvegi, G Folberth, G Ghan, SJ Horowitz, LW Lee, YH MacKenzie, IA Nagashima, T Naik, V Plummer, D Righi, M Rumbold, ST Schulz, M Skeie, RB Stevenson, DS Strode, S Sudo, K Szopa, S Voulgarakis, A Zeng, G AF Lamarque, J. -F. Shindell, D. T. Josse, B. Young, P. J. Cionni, I. Eyring, V. Bergmann, D. Cameron-Smith, P. Collins, W. J. Doherty, R. Dalsoren, S. Faluvegi, G. Folberth, G. Ghan, S. J. Horowitz, L. W. Lee, Y. H. MacKenzie, I. A. Nagashima, T. Naik, V. Plummer, D. Righi, M. Rumbold, S. T. Schulz, M. Skeie, R. B. Stevenson, D. S. Strode, S. Sudo, K. Szopa, S. Voulgarakis, A. Zeng, G. TI The Atmospheric Chemistry and Climate Model Intercomparison Project (ACCMIP): overview and description of models, simulations and climate diagnostics SO GEOSCIENTIFIC MODEL DEVELOPMENT LA English DT Article ID GENERAL-CIRCULATION MODEL; CHEMICAL-TRANSPORT MODEL; FLUX CONVECTION SCHEME; LARGE-SCALE MODELS; ACCURATE SIMULATION; CUMULUS CONVECTION; DRY DEPOSITION; NOX EMISSIONS; PARAMETERIZATION; OZONE AB The Atmospheric Chemistry and Climate Model Intercomparison Project (ACCMIP) consists of a series of time slice experiments targeting the long-term changes in atmospheric composition between 1850 and 2100, with the goal of documenting composition changes and the associated radiative forcing. In this overview paper, we introduce the ACCMIP activity, the various simulations performed (with a requested set of 14) and the associated model output. The 16 ACCMIP models have a wide range of horizontal and vertical resolutions, vertical extent, chemistry schemes and [GRAPHICA] interaction with radiation and clouds. While anthropogenic and biomass burning emissions were specified for all time slices in the ACCMIP protocol, it is found that the natural emissions are responsible for a significant range across models, mostly in the case of ozone precursors. The analysis of selected present-day climate diagnostics (precipitation, temperature, specific humidity and zonal wind) reveals biases consistent with state-of-the-art climate models. The model-to-model comparison of changes in temperature, specific humidity and zonal wind between 1850 and 2000 and between 2000 and 2100 indicates mostly consistent results. However, models that are clear outliers are different enough from the other models to significantly affect their simulation of atmospheric chemistry. C1 [Lamarque, J. -F.] Natl Ctr Atmospher Res, Earth Syst Lab, Boulder, CO 80307 USA. [Shindell, D. T.; Faluvegi, G.; Lee, Y. H.] NASA, Goddard Inst Space Studies, New York, NY 10025 USA. [Shindell, D. T.; Faluvegi, G.; Lee, Y. H.] Columbia Earth Inst, New York, NY USA. [Josse, B.] CNRS, Ctr Natl Rech Meteorol, Meteo France, GAME CNRM, Toulouse, France. [Young, P. J.] Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA. [Young, P. J.] NOAA, Div Chem Sci, Earth Syst Res Lab, Boulder, CO USA. [Cionni, I.] Agenzia Nazl Nuove Tecnol Energia & Sviluppo Econ, Bologna, Italy. [Eyring, V.; Righi, M.] Deutsch Zentrum Luft & Raumfahrt DLR, Inst Phys Atmosphare, Oberpfaffenhofen, Germany. [Bergmann, D.; Cameron-Smith, P.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Collins, W. J.; Folberth, G.; Rumbold, S. T.] Met Off, Hadley Ctr Climate Predict, Exeter, Devon, England. [Doherty, R.; MacKenzie, I. A.; Stevenson, D. S.] Univ Edinburgh, Sch Geosci, Edinburgh, Midlothian, Scotland. [Dalsoren, S.; Skeie, R. B.] CICERO, Oslo, Norway. [Ghan, S. J.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Horowitz, L. W.] NOAA, Geophys Fluid Dynam Lab, Princeton, NJ USA. [Nagashima, T.; Sudo, K.] Japan Marine Sci & Technol Ctr, Frontier Res Ctr Global Change, Yokohama, Kanagawa, Japan. [Naik, V.] UCAR NOAA, Geophys Fluid Dynam Lab, Princeton, NJ USA. [Plummer, D.] Environm Canada, Canadian Ctr Climate Modeling & Anal, Victoria, BC, Canada. [Schulz, M.] Inst Meteorol, Oslo, Norway. [Strode, S.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Strode, S.] Univ Space Res Assoc, Columbia, MD USA. [Szopa, S.] CEA CNRS UVSQ IPSL, Lab Sci Climat & Environm, Gif Sur Yvette, France. [Voulgarakis, A.] Univ London Imperial Coll Sci Technol & Med, Dept Phys, London, England. [Zeng, G.] Natl Inst Water & Atmospher Res, Lauder, New Zealand. RP Lamarque, JF (reprint author), Natl Ctr Atmospher Res, Earth Syst Lab, POB 3000, Boulder, CO 80307 USA. EM lamar@ucar.edu RI Schulz, Michael/A-6930-2011; Strode, Sarah/H-2248-2012; Ghan, Steven/H-4301-2011; Eyring, Veronika/O-9999-2016; Manager, CSD Publications/B-2789-2015; Collins, William/A-5895-2010; mackenzie, ian/E-9320-2013; Stevenson, David/C-8089-2012; Bergmann, Daniel/F-9801-2011; Young, Paul/E-8739-2010; Righi, Mattia/I-5120-2013; Cameron-Smith, Philip/E-2468-2011; Szopa, Sophie/F-8984-2010; Shindell, Drew/D-4636-2012; Horowitz, Larry/D-8048-2014; Naik, Vaishali/A-4938-2013; Lamarque, Jean-Francois/L-2313-2014; Skeie, Ragnhild/K-1173-2015; OI Schulz, Michael/0000-0003-4493-4158; Strode, Sarah/0000-0002-8103-1663; Ghan, Steven/0000-0001-8355-8699; Eyring, Veronika/0000-0002-6887-4885; Folberth, Gerd/0000-0002-1075-440X; Righi, Mattia/0000-0003-3827-5950; Collins, William/0000-0002-7419-0850; Stevenson, David/0000-0002-4745-5673; Bergmann, Daniel/0000-0003-4357-6301; Young, Paul/0000-0002-5608-8887; Cameron-Smith, Philip/0000-0002-8802-8627; Szopa, Sophie/0000-0002-8641-1737; Horowitz, Larry/0000-0002-5886-3314; Naik, Vaishali/0000-0002-2254-1700; Lamarque, Jean-Francois/0000-0002-4225-5074; Skeie, Ragnhild/0000-0003-1246-4446; Lee, Yunha/0000-0001-7478-2672 FU NASA MAP; ACMAP programs; US Department of Energy Office of Science Decadal and Regional Climate Prediction using Earth System Models (EaSM) program; DOE by Battelle Memorial Institute [DE-AC06-76RLO 1830]; US Dept. of Energy (BER); LLNL [DE-AC52-07NA27344]; NERSC [DE-AC02-05CH11231]; DLR Earth System Model Validation Project (ESMVal); German Climate Computing Center (DKRZ); ENEA National Integrated Model; Joint DECC; Defra Integrated Climate Programme [GA01101]; New Zealand Ministry of Science and Innovation; NASA Modeling, Analysis and Prediction program; UK research council grant [NE/I008063/1]; National Science Foundation; Office of Science (BER) of the US Department of Energy FX ACCMIP is organized under the auspices of Atmospheric Chemistry and Climate (AC&C), a project of International Global Atmospheric Chemistry (IGAC) and Stratospheric Processes And their Role in Climate (SPARC) under the International Geosphere-Biosphere Project (IGBP) and World Climate Research Program (WCRP). The authors are grateful to the British Atmospheric Data Centre (BADC), which is part of the NERC National Centre for Atmospheric Science (NCAS), for collecting and archiving the ACCMIP data. D. S., G. F. and Y. L. acknowledge support from the NASA MAP and ACMAP programs. D. P. would like to thank the Canadian Foundation for Climate and Atmospheric Sciences for their long-running support of CMAM development. S. G. was supported by the US Department of Energy Office of Science Decadal and Regional Climate Prediction using Earth System Models (EaSM) program. The Pacific Northwest National Laboratory (PNNL) is operated for the DOE by Battelle Memorial Institute under contract DE-AC06-76RLO 1830. The work of D. B. and P. C. was funded by the US Dept. of Energy (BER), performed under the auspices of LLNL under Contract DE-AC52-07NA27344, and used the supercomputing resources of NERSC under contract No. DE-AC02-05CH11231. V. E. and M. R. were supported by the DLR Earth System Model Validation Project (ESMVal) and used the supercomputing resources of the German Climate Computing Center (DKRZ) and the Leibniz Supercomputing Centre (LRZ) for the EMAC simulations. The work of I. C. was funded by the ENEA National Integrated Model to support the international negotiation on atmospheric pollution (Minni) project. W. J. C., G. A. F. and S. T. R. were supported by the Joint DECC and Defra Integrated Climate Programme (GA01101). V. N. and L. W. H. acknowledge efforts of GFDL's Global Atmospheric Model Development Team in the development of the GFDL-AM3 and Modeling Services Group for assistance with data processing. G. Z. acknowledges NIWA HPCF facility and funding from New Zealand Ministry of Science and Innovation. The GEOSCCM work was supported by the NASA Modeling, Analysis and Prediction program, with computing resources provided by NASA's High-End Computing Program through the NASA Advanced Supercomputing Division. The STOC-HadAM3 work was supported by cross UK research council grant NE/I008063/1 and used facilities provided by the UK's national high-performance computing service, HECToR, through Computational Modelling Services (CMS), part of the NERC National Centre for Atmospheric Science (NCAS). The LMDz-OR-INCA simulations were done using computing resources provided by the CCRT/GENCI computer center of the CEA. The MIROC-CHEM calculations were performed on the NIES supercomputer system (NEC SX-8R), and supported by the Environment Research and Technology Development Fund (S-7) of the Ministry of the Environment, Japan. The CICERO-OsloCTM2 simulations were done within the projects SLAC (Short Lived Atmospheric Components) and EarthClim funded by the Norwegian Research Council. The MOCAGE simulations were supported by Meteo-France and CNRS. Supercomputing time was provided by Meteo-France/DSI supercomputing center. The CESM project (which includes CESM-CAM-Superfast, NCAR-CAM3.5 and NCAR-CAM5.1) is supported by the National Science Foundation and the Office of Science (BER) of the US Department of Energy. The National Center for Atmospheric Research is operated by the University Corporation for Atmospheric Research under sponsorship of the National Science Foundation. NR 91 TC 113 Z9 119 U1 4 U2 73 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1991-959X EI 1991-9603 J9 GEOSCI MODEL DEV JI Geosci. Model Dev. PY 2013 VL 6 IS 1 BP 179 EP 206 DI 10.5194/gmd-6-179-2013 PG 28 WC Geosciences, Multidisciplinary SC Geology GA 118FI UT WOS:000317008500012 ER PT J AU Kirkevag, A Iversen, T Seland, O Hoose, C Kristjansson, JE Struthers, H Ekman, AML Ghan, S Griesfeller, J Nilsson, ED Schulz, M AF Kirkevag, A. Iversen, T. Seland, O. Hoose, C. Kristjansson, J. E. Struthers, H. Ekman, A. M. L. Ghan, S. Griesfeller, J. Nilsson, E. D. Schulz, M. TI Aerosol-climate interactions in the Norwegian Earth System Model-NorESM1-M SO GEOSCIENTIFIC MODEL DEVELOPMENT LA English DT Article ID COMMUNITY ATMOSPHERE MODEL; SECONDARY ORGANIC AEROSOL; BIOMASS BURNING EMISSIONS; CHEMICAL-TRANSPORT MODEL; CARBONACEOUS AEROSOLS; CLOUD MICROPHYSICS; OPTICAL-THICKNESS; MARINE AEROSOL; BLACK CARBON; ARCTIC-OCEAN AB The objective of this study is to document and evaluate recent changes and updates to the module for aerosols and aerosol-cloud-radiation interactions in the atmospheric module CAM4-Oslo of the core version of the Norwegian Earth System Model (NorESM), NorESM1-M. Particular attention is paid to the role of natural organics, sea salt, and mineral dust in determining the gross aerosol properties as well as the anthropogenic contribution to these properties and the associated direct and indirect radiative forcing. The aerosol module is extended from earlier versions that have been published, and includes life-cycling of sea salt, mineral dust, particulate sulphate, black carbon, and primary and secondary organics. The impacts of most of the numerous changes since previous versions are thoroughly explored by sensitivity experiments. The most important changes are: modified prognostic sea salt emissions; updated treatment of precipitation scavenging and gravitational settling; inclusion of biogenic primary organics and methane sulphonic acid (MSA) from oceans; almost doubled production of land-based biogenic secondary organic aerosols (SOA); and increased ratio of organic matter to organic carbon (OM/OC) for biomass burning aerosols from 1.4 to 2.6. Compared with in situ measurements and remotely sensed data, the new treatments of sea salt and dust aerosols give smaller biases in near-surface mass concentrations and aerosol optical depth than in the earlier model version. The model biases for mass concentrations are approximately unchanged for sulphate and BC. The enhanced levels of modeled OM yield improved overall statistics, even though OM is still underestimated in Europe and overestimated in North America. The global anthropogenic aerosol direct radiative forcing (DRF) at the top of the atmosphere has changed from a small positive value to -0.08 W m(-2) in CAM4-Oslo. The sensitivity tests suggest that this change can be attributed to the new treatment of biomass burning aerosols and gravitational settling. Although it has not been a goal in this study, the new DRF estimate is closer both to the median model estimate from the AeroCom intercomparison and the best estimate in IPCC AR4. Estimated DRF at the ground surface has increased by ca. 60 %, to -1.89 W m(-2). We show that this can be explained by new emission data and omitted mixing of constituents between updrafts and downdrafts in convective clouds. The increased abundance of natural OM and the introduction of a cloud droplet spectral dispersion formulation are the most important contributions to a considerably decreased estimate of the indirect radiative forcing (IndRF). The IndRF is also found to be sensitive to assumptions about the coating of insoluble aerosols by sulphate and OM. The IndRF of -1.2 W m(-2), which is closer to the IPCC AR4 estimates than the previous estimate of -1.9 W m(-2), has thus been obtained without imposing unrealistic artificial lower bounds on cloud droplet number concentrations. C1 [Kirkevag, A.; Iversen, T.; Seland, O.; Griesfeller, J.; Schulz, M.] Norwegian Meteorol Inst, Oslo, Norway. [Iversen, T.; Hoose, C.; Kristjansson, J. E.] Univ Oslo, Dept Geosci, Oslo, Norway. [Hoose, C.] Karlsruhe Inst Technol, Inst Meteorol & Climate Res, D-76021 Karlsruhe, Germany. [Struthers, H.; Nilsson, E. D.] Stockholm Univ, Dept Appl Environm Sci, S-10691 Stockholm, Sweden. [Struthers, H.; Ekman, A. M. L.] Stockholm Univ, Dept Meteorol, S-10691 Stockholm, Sweden. [Ghan, S.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Kirkevag, A (reprint author), Norwegian Meteorol Inst, Oslo, Norway. EM alf.kirkevag@met.no RI Hoose, Corinna/A-4295-2009; Schulz, Michael/A-6930-2011; Ghan, Steven/H-4301-2011 OI Hoose, Corinna/0000-0003-2827-5789; Schulz, Michael/0000-0003-4493-4158; Ghan, Steven/0000-0001-8355-8699 FU Research Council of Norway [207711/E10]; Norwegian Space Centre through PM-VRAE; EU; US Department of Energy (DOE), Office of Science, Scientific Discovery through Advanced Computing (SciDAC) Program; Office of Science Earth System Modeling Program; Battelle Memorial Institute [AC06-76RLO 1830] FX We are deeply grateful to NCAR for providing early access to model code for CCSM/CESM and to NCAR staff for invaluable advice. NorESM has benefited from contributions by many scientists at member institutions of The Norwegian Climate Centre: BCCR, met. no, MetOs-UiO, NERSC, Cicero, NILU and NP; from NCAR and PNNL in USA, and MISU and The Bolin Centre in Sweden. We are grateful to the AeroCom community for valuable discussions and for making AeroCom model intercomparison and observation data available on the AeroCom web page (http://aerocom.met.no). Thanks also to Dirk Olivie, Svetlana Tsyro, Leonor Tarrason, Hilde Fagerli, David Simpson and Brigitte Koffi for valuable discussions, and to Birthe Steensen for work with the CALIOP figures. The CALIOP data were prepared by Brigitte Koffi. This work has been supported by the Research Council of Norway through the NorClim, EarthClim (207711/E10) and NOTUR/NorStore projects, by the Norwegian Space Centre through PM-VRAE, and through the EU projects PEGASOS and ACCESS. A. Ekman, E. D. Nilsson and H. Struthers would like to acknowledge the support from the Swedish Research Council, project GRACE, and the Bert Bolin Climate Center. S. Ghan was funded by the US Department of Energy (DOE), Office of Science, Scientific Discovery through Advanced Computing (SciDAC) Program and by the Office of Science Earth System Modeling Program. The Pacific Northwest National Laboratory is operated for DOE by Battelle Memorial Institute under contract DE-AC06-76RLO 1830. NR 102 TC 56 Z9 58 U1 3 U2 44 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1991-959X J9 GEOSCI MODEL DEV JI Geosci. Model Dev. PY 2013 VL 6 IS 1 BP 207 EP 244 DI 10.5194/gmd-6-207-2013 PG 38 WC Geosciences, Multidisciplinary SC Geology GA 118FI UT WOS:000317008500013 ER PT J AU Long, MS Keene, WC Easter, R Sander, R Kerkweg, A Erickson, D Liu, X Ghan, S AF Long, M. S. Keene, W. C. Easter, R. Sander, R. Kerkweg, A. Erickson, D. Liu, X. Ghan, S. TI Implementation of the chemistry module MECCA (v2.5) in the modal aerosol version of the Community Atmosphere Model component (v3.6.33) of the Community Earth System Model SO GEOSCIENTIFIC MODEL DEVELOPMENT LA English DT Article ID MARINE BOUNDARY-LAYER; CONSISTENT SIMULATION; TECHNICAL NOTE; BROMINE CHEMISTRY; GEOS-CHEM; STRATOSPHERE; SOLVERS AB A coupled atmospheric chemistry and climate system model was developed using the modal aerosol version of the National Center for Atmospheric Research Community Atmosphere Model (modal-CAM; v3.6.33) and the Max Planck Institute for Chemistry's Module Efficiently Calculating the Chemistry of the Atmosphere (MECCA; v2.5) to provide enhanced resolution of multiphase processes, particularly those involving inorganic halogens, and associated impacts on atmospheric composition and climate. Three Rosenbrock solvers (Ros-2, Ros-3, RODAS-3) were tested in conjunction with the basic load-balancing options available to modal-CAM (1) to establish an optimal configuration of the implicitly-solved multiphase chemistry module that maximizes both computational speed and repeatability of Ros2 and RODAS-3 results versus Ros-3, and (2) to identify potential implementation strategies for future versions of this and similar coupled systems. RODAS-3 was faster than Ros-2 and Ros-3 with good reproduction of Ros-3 results, while Ros-2 was both slower and substantially less reproducible relative to Ros-3 results. Modal-CAM with MECCA chemistry was a factor of 15 slower than modal-CAM using standard chemistry. MECCA chemistry integration times demonstrated a systematic frequency distribution for all three solvers, and revealed that the change in run-time performance was due to a change in the frequency distribution of chemical integration times; the peak frequency was similar for all solvers. This suggests that efficient chemistry-focused load-balancing schemes can be developed that rely on the parameters of this frequency distribution. C1 [Long, M. S.] Harvard Univ, Sch Engn & Appl Sci, Cambridge, MA 02138 USA. [Keene, W. C.] Univ Virginia, Dept Environm Sci, Charlottesville, VA 22904 USA. [Easter, R.; Liu, X.; Ghan, S.] Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. [Sander, R.] Max Planck Inst Chem, Air Chem Dept, D-55020 Mainz, Germany. [Kerkweg, A.] Johannes Gutenberg Univ Mainz, Inst Atmospher Phys, D-55099 Mainz, Germany. [Erickson, D.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN USA. RP Long, MS (reprint author), Harvard Univ, Sch Engn & Appl Sci, Cambridge, MA 02138 USA. EM mlong@seas.harvard.edu RI Sander, Rolf/A-5725-2011; Chem, GEOS/C-5595-2014; Liu, Xiaohong/E-9304-2011; Ghan, Steven/H-4301-2011 OI Sander, Rolf/0000-0001-6479-2092; Liu, Xiaohong/0000-0002-3994-5955; Ghan, Steven/0000-0001-8355-8699 FU US Department of Energy's (DOE's) Office of Science through the Office of Biological and Environmental Research (BER) [DE-FG02-07ER64442, DE-SC0007120]; Global Change Education Program Graduate Research Environmental Fellowship; National Center for Computational Sciences at Oak Ridge National Laboratory; DOE's Office of Science (BER) [DE-AC05-00OR22725]; National Science Foundation; DOE's Office of Science (BER); US Department of Energy, Office of Science, Scientific Discovery through Advanced Computing (SciDAC) Program; DOE by Battelle Memorial Institute [DE-AC06-76RLO 1830] FX Financial support was provided by the US Department of Energy's (DOE's) Office of Science through the Office of Biological and Environmental Research (BER, grant numbers DE-FG02-07ER64442 and DE-SC0007120 to the University of Virginia), a Global Change Education Program Graduate Research Environmental Fellowship, and the National Center for Computational Sciences at Oak Ridge National Laboratory, which is supported by DOE's Office of Science (BER) under contract DE-AC05-00OR22725. The CESM project is supported by the National Science Foundation and the DOE's Office of Science (BER). PNNL authors were funded by the US Department of Energy, Office of Science, Scientific Discovery through Advanced Computing (SciDAC) Program. The Pacific Northwest National Laboratory is operated for DOE by Battelle Memorial Institute under contract DE-AC06-76RLO 1830. NR 23 TC 2 Z9 2 U1 0 U2 15 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1991-959X J9 GEOSCI MODEL DEV JI Geosci. Model Dev. PY 2013 VL 6 IS 1 BP 255 EP 262 DI 10.5194/gmd-6-255-2013 PG 8 WC Geosciences, Multidisciplinary SC Geology GA 118FI UT WOS:000317008500015 ER PT J AU Liu, XH Xiao, P MacKinnon, SND AF Liu, Xiao Hong Xiao, Ping MacKinnon, Scott N. Dr. TI IS EFFICACY OF ACUPUNCTURE TREATMENT A WISHFUL THINKING? FUNCTIONAL TEST OF ACUPUNCTURE FOR LOWER BACK PAIN, A CLINICAL STUDY SO JOURNAL OF COGNITIVE NEUROSCIENCE LA English DT Meeting Abstract CT 20th Annual Meeting of the Cognitive-Neuroscience-Society CY APR 13-16, 2013 CL San Francisco, CA SP Cognit Neuroscience Soc C1 [Liu, Xiao Hong; MacKinnon, Scott N. Dr.] Mem Univ Newfoundland, St John, NF, Canada. [Xiao, Ping] Lawrence Berkeley Natl Lab, Berkeley, CA USA. NR 0 TC 0 Z9 0 U1 2 U2 5 PU MIT PRESS PI CAMBRIDGE PA 55 HAYWARD STREET, CAMBRIDGE, MA 02142 USA SN 0898-929X J9 J COGNITIVE NEUROSCI JI J. Cogn. Neurosci. PY 2013 SU S BP 174 EP 174 PG 1 WC Neurosciences; Psychology, Experimental SC Neurosciences & Neurology; Psychology GA 118MV UT WOS:000317030501006 ER PT J AU Oh, H Mormino, EC Jagust, WJ AF Oh, Hwamee Mormino, Elizabeth C. Jagust, William J. TI EFFECTS OF AGING AND BETA-AMYLOID DEPOSITION ON EPISODIC ENCODING BRAIN ACTIVITY IN COGNITIVELY NORMAL ELDERLY SO JOURNAL OF COGNITIVE NEUROSCIENCE LA English DT Meeting Abstract CT 20th Annual Meeting of the Cognitive-Neuroscience-Society CY APR 13-16, 2013 CL San Francisco, CA SP Cognit Neuroscience Soc C1 [Oh, Hwamee; Jagust, William J.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Mormino, Elizabeth C.] Harvard Univ, Sch Med, Cambridge, MA 02138 USA. [Jagust, William J.] Lawrence Berkeley Natl Lab, Berkeley, CA USA. NR 0 TC 0 Z9 0 U1 0 U2 1 PU MIT PRESS PI CAMBRIDGE PA 55 HAYWARD STREET, CAMBRIDGE, MA 02142 USA SN 0898-929X J9 J COGNITIVE NEUROSCI JI J. Cogn. Neurosci. PY 2013 SU S BP 226 EP 226 PG 1 WC Neurosciences; Psychology, Experimental SC Neurosciences & Neurology; Psychology GA 118MV UT WOS:000317030501251 ER PT J AU Watson, P Jane, W Neal, C AF Watson, Patrick Jane, Wang Neal, Cohen TI EVENT RECONSTRUCTION REVEALS RELATIONAL REPRESENTATIONS THAT DO NOT OVERLAP WITH THE SEMANTIC INFORMATION PRESENT IN THE EXPERIMENT SO JOURNAL OF COGNITIVE NEUROSCIENCE LA English DT Meeting Abstract CT 20th Annual Meeting of the Cognitive-Neuroscience-Society CY APR 13-16, 2013 CL San Francisco, CA SP Cognit Neuroscience Soc C1 [Watson, Patrick; Neal, Cohen] Univ Illinois, Urbana, IL 61801 USA. [Watson, Patrick] Sandia Natl Labs, Livermore, CA 94550 USA. [Jane, Wang] Northwestern Univ, Evanston, IL 60208 USA. NR 0 TC 0 Z9 0 U1 0 U2 1 PU MIT PRESS PI CAMBRIDGE PA 55 HAYWARD STREET, CAMBRIDGE, MA 02142 USA SN 0898-929X J9 J COGNITIVE NEUROSCI JI J. Cogn. Neurosci. PY 2013 SU S BP 249 EP 249 PG 1 WC Neurosciences; Psychology, Experimental SC Neurosciences & Neurology; Psychology GA 118MV UT WOS:000317030501361 ER PT J AU Vakhtin, A Calhoun, V Jung, R Prestopnik, J Taylor, P Ford, C AF Vakhtin, Andrei Calhoun, Vince Jung, Rex Prestopnik, Jillian Taylor, Paul Ford, Corey TI CHANGES IN INTRINSIC FUNCTIONAL BRAIN NETWORKS FOLLOWING BLAST-INDUCED MILD TRAUMATIC BRAIN INJURY SO JOURNAL OF COGNITIVE NEUROSCIENCE LA English DT Meeting Abstract CT 20th Annual Meeting of the Cognitive-Neuroscience-Society CY APR 13-16, 2013 CL San Francisco, CA SP Cognit Neuroscience Soc C1 [Vakhtin, Andrei; Calhoun, Vince; Jung, Rex; Prestopnik, Jillian; Ford, Corey] Univ New Mexico, Albuquerque, NM 87131 USA. [Taylor, Paul] Sandia Natl Labs, Livermore, CA 94550 USA. NR 0 TC 0 Z9 0 U1 0 U2 1 PU MIT PRESS PI CAMBRIDGE PA 55 HAYWARD STREET, CAMBRIDGE, MA 02142 USA SN 0898-929X J9 J COGNITIVE NEUROSCI JI J. Cogn. Neurosci. PY 2013 SU S BP 261 EP 261 PG 1 WC Neurosciences; Psychology, Experimental SC Neurosciences & Neurology; Psychology GA 118MV UT WOS:000317030501417 ER PT J AU Michalak, SE Hamada, MS Hengartner, NW AF Michalak, Sarah E. Hamada, Michael S. Hengartner, Nicolas W. TI Analysis of interval-censored data with random unknown end points: an application to soft error rate estimation SO JOURNAL OF THE ROYAL STATISTICAL SOCIETY SERIES C-APPLIED STATISTICS LA English DT Article DE Failure time data; Hardware reliability; Measurement error; Measurement process ID FIT AB . The paper presents a Bayesian approach to analysing interval-censored data with random unknown end points. Such data occur when the event of interest is interval censored but, because of the measurement process, the interval end points are not known exactly. Modelling the measurement process permits inference that accounts for this source of variability. Our results are motivated by an experimental study that was designed to characterize the cosmic-rayneutron-induced soft error rate of a semiconductor device. C1 [Michalak, Sarah E.; Hamada, Michael S.; Hengartner, Nicolas W.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Michalak, SE (reprint author), Los Alamos Natl Lab, Stat Sci Grp, MS F600, Los Alamos, NM 87545 USA. EM michalak@lanl.gov NR 15 TC 3 Z9 3 U1 2 U2 5 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0035-9254 J9 J R STAT SOC C-APPL JI J. R. Stat. Soc. Ser. C-Appl. Stat. PY 2013 VL 62 IS 3 BP 473 EP 486 DI 10.1111/rssc.12005 PG 14 WC Statistics & Probability SC Mathematics GA 123RW UT WOS:000317409400007 ER PT S AU Tang, M Fuierer, P Dickens, P Fu, EG AF Tang, Ming Fuierer, Paul Dickens, Peter Fu, Engang BE Stanek, C TI Irradiation study on Srn+1TinO3n+1 Ruddlesden-Popper phases synthesized by hot-forging SO PHYSICA STATUS SOLIDI C: CURRENT TOPICS IN SOLID STATE PHYSICS, VOL 10, NO 2 SE Physica Status Solidi C-Current Topics in Solid State Physics LA English DT Proceedings Paper CT 18th International Conference on Defects in Insulating Materials (ICDIM) CY JUN 24-29, 2012 CL Santa Fe, NM SP New Mexico Consortium, Los Alamos Natl Bank (LANB), Netzsch, Los Alamos Natl Lab DE Srn+1TinO3n+1; Ruddlesden-Popper; radiation damage ID POWDER DIFFRACTION; TEMPERATURE; SRTIO3; ION; CERAMICS AB The hot-forging technique was used to obtain both the n = 2 (Sr3Ti2O7) and n = infinity (SrTiO3) members of Ruddlesden-Popper phase Srn+1TinO3n+1. Pure phase and high density (>95% theoretical) materials were achieved using this technique. These polycrystalline samples were irradiated with 200 keV He ions to a fluence of 2x10(21) ion/m(2) (corresponding to a peak dose at 5 dpa) at room temperature to study radiation damage effects. Microstructural investigation on pristine and irradiated samples was performed using grazing incidence X-ray diffraction (GIXRD) and transmission electron microscopy (TEM). Three phenomena are revealed upon comparing prisXtine versus irradiated samples. First, both compounds interplanar lattice spacings increased after irradiation. Second, peak broadening possibly suggests incredibly small grain due to irradiation. Third, experiment results revealed an amorphization in the irradiated Sr3Ti2O7, while no amorphization was observed in irradiated SrTiO3. (c) 2012 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim C1 [Tang, Ming] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. RP Tang, M (reprint author), Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. EM mtang@lanl.gov NR 27 TC 4 Z9 4 U1 1 U2 11 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA PAPPELALLEE 3, W-69469 WEINHEIM, GERMANY SN 1862-6351 J9 PHYS STATUS SOLIDI C PY 2013 VL 10 IS 2 BP 216 EP 220 DI 10.1002/pssc.201200523 PG 5 WC Materials Science, Multidisciplinary; Physics, Condensed Matter SC Materials Science; Physics GA BEM08 UT WOS:000317294600015 ER PT S AU Blair, MW Fasoli, M Tornga, SC Vedda, A Smith, NA Bennett, BL Hehlen, MP Muenchausen, RE AF Blair, Michael W. Fasoli, Mauro Tornga, Stephanie C. Vedda, Anna Smith, Nickolaus A. Bennett, Bryan L. Hehlen, Markus P. Muenchausen, Ross E. BE Stanek, C TI Nanophosphor GdOBr:Ce via combustion synthesis: luminescence results SO PHYSICA STATUS SOLIDI C: CURRENT TOPICS IN SOLID STATE PHYSICS, VOL 10, NO 2 SE Physica Status Solidi C-Current Topics in Solid State Physics LA English DT Proceedings Paper CT 18th International Conference on Defects in Insulating Materials (ICDIM) CY JUN 24-29, 2012 CL Santa Fe, NM SP New Mexico Consortium, Los Alamos Natl Bank (LANB), Netzsch, Los Alamos Natl Lab DE combustion synthesis; scintillation; luminescence ID SIZE AB We used combustion synthesis to produce phase pure GdOBr:Ce with varying Ce concentration. Several combinations of NH4Br and fuel concentration were tested before phase pure GdOBr:Ce was produced by using a 50% excess of NH4Br and a 50% lean concentration of fuel. In addition to the expected emissions from Ce and Gd, we also detected emissions from Eu3+ and Tb3+. Further research indicated that these extra rare earth emissions were due to impurities in the Gd2O3 starting material. While not the desired effect, we were able to monitor both Eu and Ce intensities as a function of Ce concentration in GdOBr. The Ce emission is seen to reach a maximum between 0.1 and 0.5 mol %. At higher Ce content, the Ce luminescence is quenched because of the concentration quenching effect and the higher concentration of O-H and N-H groups as revealed by IR spectra. Eu emission progressively decreases as Ce content increases from a combination of competition with Ce for charge capture in the RL process and the effect of OH and NH groups. As Ce concentration increases the RL intensity ratio of the bands of the Ce doublet changes even though the energy difference between the two bands (0.24 +/- 0.1 eV) is compatible with the spin-orbit splitting of the ground level of Ce3+ (0.25 eV). Fitting results indicate that this relative change is not due to changes in self-absorption, and the effect may be due to changes in local symmetry of the Ce ion. (c) 2012 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim C1 [Blair, Michael W.; Tornga, Stephanie C.; Smith, Nickolaus A.; Bennett, Bryan L.; Hehlen, Markus P.; Muenchausen, Ross E.] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. RP Blair, MW (reprint author), Los Alamos Natl Lab, Div Mat Sci & Technol, POB 1663, Los Alamos, NM 87545 USA. EM mblair@lanl.gov OI Fasoli, Mauro/0000-0001-5463-4875 NR 20 TC 0 Z9 0 U1 2 U2 9 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA PAPPELALLEE 3, W-69469 WEINHEIM, GERMANY SN 1862-6351 J9 PHYS STATUS SOLIDI C PY 2013 VL 10 IS 2 BP 227 EP 231 DI 10.1002/pssc.201200525 PG 5 WC Materials Science, Multidisciplinary; Physics, Condensed Matter SC Materials Science; Physics GA BEM08 UT WOS:000317294600017 ER PT S AU Liliental-Weber, Z dos Reis, R Novikov, SV Yu, KM Levander, AX Dubon, OD Wu, J Walukiewicz, W Foxon, CT AF Liliental-Weber, Z. dos Reis, R. Novikov, S. V. Yu, K. M. Levander, A. X. Dubon, O. D. Wu, J. Walukiewicz, W. Foxon, C. T. BE Toropov, A Ivanov, S TI Microstructure of Mg doped GaNAs alloys SO PHYSICA STATUS SOLIDI C: CURRENT TOPICS IN SOLID STATE PHYSICS, VOL 10, NO 3 SE Physica Status Solidi C-Current Topics in Solid State Physics LA English DT Proceedings Paper CT 4th International Symposium on Growth of III-Nitrides (ISGN) CY JUL 16-19, 2012 CL Saint-Petersburg, RUSSIA SP Russian Acad Sci, Ioffe Phys-Tech Inst, Riber, Aixtron, Komef, U S Army Foward Element Commmand Atlantic, Off Naval Res Sci & Technol, SemiTEq, Veeco, Optogan LED Solut, Crystal IS DE nitride semiconductors; p-doping; TEM; amorphous materials; planar defect; conductivity AB Transmission Electron Microscopy of Mg doped GaN1-xAsx samples, grown by MBE at low temperatures, show substantial structural changes for samples that are semi-insulating and those with high or low conductivity. The conductive samples show p-type conductivity as evidence from the positive thermopower values. All the Mg doped samples show phase segregation: cubic GaAs and GaN grains (a mixture of cubic and some hexagonal) phases within an amorphous matrix. The best conductive samples show cubic GaAs grains with high density of stacking faults embedded into an amorphous matrix. The samples that are less conductive have lower ratio of the amorphous to the crystalline phase of the samples and much lower density of stacking faults. Higher Mg concentration is expected in the amorphous parts of the samples The semi-insulating samples that have either low Mg concentration or low As show grains of GaAs and GaN attached to each other with no evidence of the amorphous phase between them. There are no SFs in these grains. It is possible that the presence of the GaN between the GaAs grains lead to semi-insulating material properties since p-type doping of GaN is more difficult. (C) 2012 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim C1 [Liliental-Weber, Z.; dos Reis, R.; Yu, K. M.; Levander, A. X.; Dubon, O. D.; Wu, J.; Walukiewicz, W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, M-S 62R203-8255, Berkeley, CA 94720 USA. [Foxon, C. T.] Univ Nottingham, Sch Phys & Astron, Nottingham NG7 2RD, England. [Levander, A. X.; Dubon, O. D.; Wu, J.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. RP Liliental-Weber, Z (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, M-S 62R203-8255, Berkeley, CA 94720 USA. EM z_liliental-weber@lbl.gov RI Wu, Junqiao/G-7840-2011; Foundry, Molecular/G-9968-2014; OI Wu, Junqiao/0000-0002-1498-0148; Yu, Kin Man/0000-0003-1350-9642 FU Director, Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Director, Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The authors appreciate the use of the TEM facility at the National Center for Electron Microscopy at the Lawrence Berkeley National Laboratory. NR 12 TC 0 Z9 0 U1 1 U2 11 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA PAPPELALLEE 3, W-69469 WEINHEIM, GERMANY SN 1862-6351 J9 PHYS STATUS SOLIDI C PY 2013 VL 10 IS 3 BP 453 EP 456 DI 10.1002/pssc.201200666 PG 4 WC Materials Science, Multidisciplinary; Physics, Condensed Matter SC Materials Science; Physics GA BEM01 UT WOS:000317290800043 ER PT J AU Tian, H Yang, Y Xie, D Ren, TL Shu, Y Sun, H Zhou, CJ Liu, X Tao, LQ Ge, J Zhang, CH Zhang, YG AF Tian, He Yang, Yi Xie, Dan Ren, Tian-Ling Shu, Yi Sun, Hui Zhou, Chang-Jian Liu, Xuan Tao, Lu-Qi Ge, Jie Zhang, Cang-Hai Zhang, Yuegang TI Laser directed lithography of asymmetric graphene ribbons on a polydimethylsiloxane trench structure SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID SINGLE-LAYER GRAPHENE; THERMAL-CONDUCTIVITY; EXFOLIATED GRAPHENE; RAMAN-SPECTROSCOPY; MONOLAYER GRAPHENE; RESONATORS; TRANSISTOR; FILMS; OXIDE AB Recently, manipulating heat transport by asymmetric graphene ribbons has received significant attention, in which phonons in the carbon lattice are used to carry energy. In addition to heat control, asymmetric graphene ribbons might also have broad applications in renewable energy engineering, such as thermoelectric energy harvesting. Here, we transfer a single sheet of graphene over a 5 mu m trench of polydimethylsiloxane (PDMS) structure. By using a laser (1.77 mW, 1 mu m diameter spot size, 517 nm wavelength) focusing on one side of the suspended graphene, a triangular shaped graphene ribbon is obtained. As the graphene has a negative thermal expansion coefficient, local laser heating could make the affected graphene area shrink and eventually break. Theoretical calculation shows that the 1.77 mW laser could create a local hot spot as high as 1462.5 degrees C, which could induce an asymmetric shape structure. We also find the temperature coefficient (-13.06 cm(-1) mW) of suspended graphene on PDMS trench substrate is ten times higher than that reported on SiO2/Si trench substrate. Collectively, our results raise the exciting prospect that the realization of graphene with asymmetric shape on thermally insulating substrate is technologically feasible, which may open up important applications in thermal circuits and thermal management. C1 [Tian, He; Yang, Yi; Xie, Dan; Ren, Tian-Ling; Shu, Yi; Sun, Hui; Zhou, Chang-Jian; Liu, Xuan; Tao, Lu-Qi; Ge, Jie; Zhang, Cang-Hai] Tsinghua Univ, Tsinghua Natl Lab Informat Sci & Technol TNList, Inst Microelect, Beijing 100084, Peoples R China. [Zhang, Yuegang] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. RP Ren, TL (reprint author), Tsinghua Univ, Tsinghua Natl Lab Informat Sci & Technol TNList, Inst Microelect, Beijing 100084, Peoples R China. EM RenTL@tsinghua.edu.cn; yzhang5@lbl.gov RI Tian, He/I-1299-2014; Zhang, Y/E-6600-2011; Foundry, Molecular/G-9968-2014 OI Tian, He/0000-0001-7328-2182; Zhang, Y/0000-0003-0344-8399; FU National Natural Science Foundation of China [61025021, 60936002, 51072089, 61020106006]; National Key Project of Science and Technology [2011ZX02403-002]; Office of Science, Office of Basic Energy Sciences, of the U. S. Department of Energy [DE-AC02-05CH11231]; Ministry of Education Scholarship of China FX This work was supported by the National Natural Science Foundation of China (61025021, 60936002, 51072089, and 61020106006), the National Key Project of Science and Technology (2011ZX02403-002). The graphene sample preparation, optical and Raman characterizations of the graphene devices were performed at the Molecular Foundry of Lawrence Berkeley National Laboratory, supported by the Office of Science, Office of Basic Energy Sciences, of the U. S. Department of Energy under contract no. DE-AC02-05CH11231. H. Tian is additionally supported by the Ministry of Education Scholarship of China. We are grateful for the PDMS trench structure prepared by D. Wang from Lawrence Berkeley National Laboratory and helpful discussion with G. Zhang from Peking University. NR 37 TC 2 Z9 2 U1 3 U2 58 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PY 2013 VL 15 IS 18 BP 6825 EP 6830 DI 10.1039/c3cp50538c PG 6 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 129TU UT WOS:000317866300030 PM 23545537 ER PT J AU Wang, B Richardson, TJ Chen, GY AF Wang, Bin Richardson, Thomas J. Chen, Guoying TI Stable and high-rate overcharge protection for rechargeable lithium batteries SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID REDOX SHUTTLE ADDITIVES; LI-ION CELLS; ELECTROACTIVE POLYMERS; PERFORMANCE AB Rechargeable lithium or lithium-ion cells can be overcharge-protected by an electroactive polymer composite separator. The use of non-woven fibrous membranes instead of conventional microporous membranes as the composite substrates allowed better distribution of the electroactive polymer, which led to improved utilization and a 40-fold increase in sustainable current density. For the first time, stable overcharge protection for hundreds of cycles was demonstrated in several cell chemistries, including LiNi1/3Co1/3Mn1/3O2, LiFePO4, and spinel Li1.05Mn1.95O4 half-cells. Protection at a charging rate as high as 5 C was achieved at a steady state cell potential below 4.85 V. C1 [Wang, Bin; Richardson, Thomas J.; Chen, Guoying] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. RP Chen, GY (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. EM gchen@lbl.gov RI Wang, Bin/F-9677-2012 OI Wang, Bin/0000-0001-7104-4543 FU Office of FreedomCAR and Vehicle Technologies of the U. S. Department of Energy [DE-AC02-05CH11231] FX We thank Dr Wei Zhang for assisting with electrode fabrication. This work was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of FreedomCAR and Vehicle Technologies of the U. S. Department of Energy under contract no. DE-AC02-05CH11231. NR 21 TC 4 Z9 4 U1 4 U2 85 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PY 2013 VL 15 IS 18 BP 6849 EP 6855 DI 10.1039/c3cp50992c PG 7 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 129TU UT WOS:000317866300033 PM 23545568 ER PT J AU McDermott, D Amelang, J Lopatina, LM Reichhardt, CJO Reichhardt, C AF McDermott, Danielle Amelang, Jeff Lopatina, Lena M. Reichhardt, Cynthia J. Olson Reichhardt, Charles TI Domain and stripe formation between hexagonal and square ordered fillings of colloidal particles on periodic pinning substrates SO SOFT MATTER LA English DT Article ID GROUND-STATES; ARRAYS; COMMENSURATE; CRYSTALS; MONOLAYERS; DEFECTS; SYSTEMS; LATTICE; DRIVEN; FIELDS AB Using large scale numerical simulations, we examine the ordering of colloidal particles on square periodic two-dimensional muffin-tin substrates consisting of a flat surface with localized pinning sites. We show that when there are four particles per pinning site, the particles adopt a hexagonal ordering, while for five particles per pinning site, a square ordering appears. For fillings between four and five particles per pinning site, we identify a rich variety of distinct ordering regimes, including disordered grain boundaries, crystalline stripe structures, superlattice orderings, and disordered patchy arrangements. We characterize the different regimes using Voronoi analysis, energy dispersion, and ordering of the domains. We show that many of the boundary formation features we observe occur for a wide range of other fillings. Our results demonstrate that grain boundary tailoring can be achieved with muffin-tin periodic pinning substrates. C1 [McDermott, Danielle; Amelang, Jeff; Lopatina, Lena M.; Reichhardt, Cynthia J. Olson; Reichhardt, Charles] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [McDermott, Danielle] Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. [Amelang, Jeff] CALTECH, Div Engn & Appl Sci, Pasadena, CA 91125 USA. RP Reichhardt, CJO (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM cjrx@lanl.gov FU NNSA of the U.S. DoE at LANL [DE-AC52-06NA25396]; ASC Summer Workshop program at LANL FX This work was carried out under the auspices of the NNSA of the U.S. DoE at LANL under Contract no. DE-AC52-06NA25396. D. M. and J.A. received support from the ASC Summer Workshop program at LANL. NR 33 TC 11 Z9 11 U1 2 U2 11 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1744-683X J9 SOFT MATTER JI Soft Matter PY 2013 VL 9 IS 18 BP 4607 EP 4613 DI 10.1039/c3sm27652j PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary; Physics, Multidisciplinary; Polymer Science SC Chemistry; Materials Science; Physics; Polymer Science GA 124WL UT WOS:000317499000006 ER PT J AU Kipnusu, WK Kossack, W Iacob, C Zeigermann, P Jasiurkowska, M Sangoro, JR Valiullin, R Kremer, F AF Kipnusu, Wycliffe Kiprop Kossack, Wilhelm Iacob, Ciprian Zeigermann, Philipp Jasiurkowska, Malgorzata Sangoro, Joshua Rume Valiullin, Rustem Kremer, Friedrich TI The interplay between inter- and intra-molecular dynamics in a series of alkylcitrates SO SOFT MATTER LA English DT Article ID GLASS-TRANSITION; HYDROGEN-BONDS; LIQUIDS AB The inter- and intra-molecular dynamics in a series of glass-forming alkylcitrates is studied by a combination of Broadband Dielectric Spectroscopy (BDS), Pulsed Field Gradient Nuclear Magnetic Resonance (PFG NMR), Fourier-Transform Infrared (FTIR) spectroscopy and Differential Scanning Calorimetry (DSC). Analyzing the temperature dependencies of specific IR absorption bands in terms of their spectral position and the corresponding oscillator strengths enables one to unravel the intramolecular dynamics of specific molecular moieties and to compare them with the (primarily dielectrically) determined intermolecular dynamics. With decreasing temperature, the IR band positions of carbonyls (part of the core units) and H-bonded moieties of citrates show a red shift with a kink at the calorimetric glass transition temperature (T-g) while other moieties, whose dynamics are decoupled from those of the core units, exhibit a blue shift with nominal changes at T-g. The oscillator strength of all units in citrates depicts stronger temperature dependencies above T-g and in some, the ester linkage and H-bonded units show a change of slope at a temperature where structural and faster secondary relaxations merge. By that, a wealth of novel information is obtained proving the fundamental importance of intramolecular mobility in the process of glass formation, beyond coarse-grained descriptions. C1 [Kipnusu, Wycliffe Kiprop; Kossack, Wilhelm; Iacob, Ciprian; Zeigermann, Philipp; Jasiurkowska, Malgorzata; Valiullin, Rustem; Kremer, Friedrich] Univ Leipzig, Inst Expt Phys 1, D-04103 Leipzig, Germany. [Sangoro, Joshua Rume] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37830 USA. RP Kipnusu, WK (reprint author), Univ Leipzig, Inst Expt Phys 1, Linnestr 5, D-04103 Leipzig, Germany. EM Kipnusu@physik.uni-leipzig.de RI Valiullin, Rustem/F-6432-2011; Iacob, Ciprian/Q-7812-2016; Sangoro, Joshua/A-6573-2011; OI Sangoro, Joshua/0000-0002-5483-9528; Kiprop Kipnusu, Wycliffe/0000-0003-0643-7716; Kossack, Wilhelm/0000-0003-1578-8454 FU DFG (Germany); NOW (The Netherlands) within IRTG 'Diffusion in Porous Materials'; Leipzig School of Natural Sciences, 'Building with Molecules and Nano-Objects' (BuilMoNa) FX Financial support from DFG (Germany) and NOW (The Netherlands) within IRTG 'Diffusion in Porous Materials' and Leipzig School of Natural Sciences, 'Building with Molecules and Nano-Objects' (BuilMoNa) is gratefully acknowledged. We also thank Dr Thomas Lupke of Kunststoff-Zentrum in Leipzig for carrying out DSC measurements. NR 25 TC 10 Z9 10 U1 1 U2 22 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1744-683X J9 SOFT MATTER JI Soft Matter PY 2013 VL 9 IS 18 BP 4681 EP 4686 DI 10.1039/c3sm27670h PG 6 WC Chemistry, Physical; Materials Science, Multidisciplinary; Physics, Multidisciplinary; Polymer Science SC Chemistry; Materials Science; Physics; Polymer Science GA 124WL UT WOS:000317499000016 ER PT S AU Pereira, H Lettry, J Alessi, J Kalvas, T AF Pereira, H. Lettry, J. Alessi, J. Kalvas, T. BE Tarvainen, O Kalvas, T TI Estimation of Sputtering Damages on a Magnetron H- Ion Source Induced by Cs+ and H+ Ions SO THIRD INTERNATIONAL SYMPOSIUM ON NEGATIVE IONS, BEAMS AND SOURCES (NIBS 2012) SE AIP Conference Proceedings LA English DT Proceedings Paper CT 3rd International Symposium on Negative Ions, Beams and Sources (NIBS) CY SEP 03-07, 2012 CL Jyvaskyla, FINLAND SP Dehnel - Particle Accelerator Components & Engn Inc, Federat Finnish Learned Soc, Univ Jyvaskyla, Dept Phys, Univ Jyvaskyla DE negative ion source; H-; Cesium; sputtering damages AB An H- ion source is being developed for CERN's Linac4 accelerator. A beam current requirement of 80 mA and a reliability above 99 % during 1 year with 3 month uninterrupted operation periods are mandatory. To design a low-maintenance long life-time source, it is important to investigate and understand the wear mechanisms. A cesiated plasma discharge ion source, such as the BNL magnetron source, is a good candidate for the Linac4 ion source. However, in the magnetron source operated at BNL, the removal of material from the molybdenum cathode and the stainless steel anode cover plate surfaces is visible after extended operation periods. The observed sputtering traces are shown to result from cesium vapors and hydrogen gas ionized in the extraction region and subsequently accelerated by the extraction field. This paper presents a quantitative estimate of the ionization of cesium and hydrogen by the electron and H- beams in the extraction region of BNL's magnetron ion source. The respective contributions of Cs+ and H+ ions to the sputtering process are estimated. C1 [Pereira, H.; Lettry, J.] CERN, CH-1211 Geneva 23, Switzerland. [Alessi, J.] BNL, New York, NY 11973 USA. [Kalvas, T.] Univ Jyvaskyla, Dept Phys, SF-40351 Jyvaskyla, Finland. RP Pereira, H (reprint author), CERN, CH-1211 Geneva 23, Switzerland. NR 8 TC 0 Z9 0 U1 0 U2 1 PU AMER INST PHYSICS PI MELVILLE PA 2 HUNTINGTON QUADRANGLE, STE 1NO1, MELVILLE, NY 11747-4501 USA SN 0094-243X BN 978-0-7354-1136-4 J9 AIP CONF PROC PY 2013 VL 1515 BP 81 EP 88 DI 10.1063/1.4792773 PG 8 WC Physics, Applied; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Physics GA BEK03 UT WOS:000317013500010 ER PT S AU Kashiwagi, M Taniguchi, M Umeda, N Dairaku, M Tobari, H Yamanaka, H Watanabe, K Inoue, T de Esch, HPL Grisham, LR Boilson, D Hemsworth, RS Tanaka, M AF Kashiwagi, Mieko Taniguchi, Masaki Umeda, Naotaka Dairaku, Masayuki Tobari, Hiroyuki Yamanaka, Haruhiko Watanabe, Kazuhiro Inoue, Takashi de Esch, H. P. L. Grisham, Larry R. Boilson, Deirdre Hemsworth, Ronald S. Tanaka, Masanobu BE Tarvainen, O Kalvas, T TI Compensations of beamlet deflections for 1 MeV accelerator of ITER NBI SO THIRD INTERNATIONAL SYMPOSIUM ON NEGATIVE IONS, BEAMS AND SOURCES (NIBS 2012) SE AIP Conference Proceedings LA English DT Proceedings Paper CT 3rd International Symposium on Negative Ions, Beams and Sources (NIBS) CY SEP 03-07, 2012 CL Jyvaskyla, FINLAND SP Dehnel - Particle Accelerator Components & Engn Inc, Federat Finnish Learned Soc, Univ Jyvaskyla, Dept Phys, Univ Jyvaskyla DE Negative ion; Accelerator; Ion beam; ITER; NBI AB Compensation methods of beamlet deflections have been studied in a three dimensional (3D) beam analysis using OPERA-3d code for 1 MeV accelerator of the ITER neutral beam injector (NBI). The beamlet deflection is caused by i) magnetic field generated by permanent magnets embedded in the extraction grid (EXG) for electron suppression and ii) space charge repulsion between the beamlets and beam groups. Moreover, the beamlet deflection is caused due to electric field distortion formed by a grid support structure. In order to compensate the beamlet deflections due to i) and ii), an aperture offset of 0.6 mm was applied in the electron suppression grid (ESG) and a metal bar with 3 mm in thickness, so-called a kerb, was attached around the aperture area at the back side of the ESG, respectively. Detailed configuration of the compensation methods was also considered so as to suppress the beam spread due to the electric field distortion and to lower electric field concentrations at the edge of the kerb. For the beamlets near the grid support structure, the beamlet deflection due to the space charge repulsion could be negated due to the electric field distortion formed by the grid support structure C1 [Kashiwagi, Mieko; Taniguchi, Masaki; Umeda, Naotaka; Dairaku, Masayuki; Tobari, Hiroyuki; Yamanaka, Haruhiko; Watanabe, Kazuhiro; Inoue, Takashi] Japan Atom Energy Agcy, 801-1 Mukoyama, Naka, Ibaraki 3110193, Japan. [de Esch, H. P. L.] CEA Cadarache, IRFM, F-13108 St Paul Les Durance, France. [Grisham, Larry R.] Princeton Univ, Plasma Phys Lab, Princeton, NJ 08543 USA. [Boilson, Deirdre; Hemsworth, Ronald S.; Tanaka, Masanobu] ITER Org, F-13115 St Paul Les Durance, France. RP Kashiwagi, M (reprint author), Japan Atom Energy Agcy, 801-1 Mukoyama, Naka, Ibaraki 3110193, Japan. FU ITER [C53TD48FJ] FX This report is based on work undertaken within the ITER Organization and/or its members, i.e., China, European Union, Inida, Japan, Korea, Russia and the United States of America. Disseminaation of information contained in this paper is governed by the applicable terms of the ITER agreement. The views and opinions expressed hereindo not necessarily reflect those of the ITER Organization. Part of this work was founded by ITER task contract (C53TD48FJ). NR 16 TC 5 Z9 5 U1 0 U2 4 PU AMER INST PHYSICS PI MELVILLE PA 2 HUNTINGTON QUADRANGLE, STE 1NO1, MELVILLE, NY 11747-4501 USA SN 0094-243X BN 978-0-7354-1136-4 J9 AIP CONF PROC PY 2013 VL 1515 BP 227 EP 236 DI 10.1063/1.4792789 PG 10 WC Physics, Applied; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Physics GA BEK03 UT WOS:000317013500026 ER PT S AU Stockli, MP Han, BX Murray, SN Pennisi, TR Santana, M Welton, RF AF Stockli, Martin P. Han, B. X. Murray, S. N. Pennisi, T. R. Santana, M. Welton, R. F. BE Tarvainen, O Kalvas, T TI Recent Performance of the SNS H- Source for 1-MW Neutron Production SO THIRD INTERNATIONAL SYMPOSIUM ON NEGATIVE IONS, BEAMS AND SOURCES (NIBS 2012) SE AIP Conference Proceedings LA English DT Proceedings Paper CT 3rd International Symposium on Negative Ions, Beams and Sources (NIBS) CY SEP 03-07, 2012 CL Jyvaskyla, FINLAND SP Dehnel - Particle Accelerator Components & Engn Inc, Federat Finnish Learned Societies, Univ Jyvaskyla, Dept Phys, Univ Jyvaskyla DE Cesium; H- ions; ion source; RF ion source; multicusp ion source ID ION-SOURCE; DESIGN AB This paper describes the performance of the SNS H- ion source and LEBT as they continue to deliver similar to 50 mA H- beams at a 5.3% duty factor required for neutron production with a similar to 1MW proton beam since the fall of 2009. The source continues to deliver persistent H- beams for up to 6 weeks without adding Cs after an initial dose of similar to 4 mg, except when there are excessive plasma impurities. In one case the H- beam decayed due to an air leak, which is shown to be consistent with sputtering of the Cs layer, and which allows us to bracket the plasma potential. In another case, the performance of two sources degraded progressively, which appears to be consistent with a progressive deterioration of the Cs covered Mo converter. These two and other recently discovered issues are discussed in detail. C1 [Stockli, Martin P.; Han, B. X.; Murray, S. N.; Pennisi, T. R.; Santana, M.; Welton, R. F.] Oak Ridge Natl Lab, Spallat Neutron Source, Oak Ridge, TN 37831 USA. RP Stockli, MP (reprint author), Oak Ridge Natl Lab, Spallat Neutron Source, Oak Ridge, TN 37831 USA. NR 16 TC 5 Z9 5 U1 0 U2 1 PU AMER INST PHYSICS PI MELVILLE PA 2 HUNTINGTON QUADRANGLE, STE 1NO1, MELVILLE, NY 11747-4501 USA SN 0094-243X BN 978-0-7354-1136-4 J9 AIP CONF PROC PY 2013 VL 1515 BP 292 EP 301 DI 10.1063/1.4792797 PG 10 WC Physics, Applied; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Physics GA BEK03 UT WOS:000317013500034 ER PT S AU Bollinger, DS AF Bollinger, D. S. BE Tarvainen, O Kalvas, T TI H- Ion Source Development for the FNAL 750keV Injector Upgrade SO THIRD INTERNATIONAL SYMPOSIUM ON NEGATIVE IONS, BEAMS AND SOURCES (NIBS 2012) SE AIP Conference Proceedings LA English DT Proceedings Paper CT 3rd International Symposium on Negative Ions, Beams and Sources (NIBS) CY SEP 03-07, 2012 CL Jyvaskyla, FINLAND SP Dehnel - Particle Accelerator Components & Engn Inc, Federat Finnish Learned Societies, Univ Jyvaskyla, Dept Phys, Univ Jyvaskyla DE Ion Source; Magnetron; RFQ; HINS; Cockcroft-Walton AB The new FNAL 750keV injector upgrade for the replacement of the 40 year old Fermi National Laboratory (FNAL) Cockcroft-Walton accelerators with a new ion source and 200MHz Radio Frequency Quadrupole (RFQ), Low Energy Beam Transport (LEBT) and Medium Energy Beam Transport (MEBT) [1], has been built and is now being tested prior to installation during the 2012 shutdown. The new H -ion source is a round aperture magnetron which was developed at Brookhaven National Lab (BNL) by Jim Alessi[2]. Operational experience from BNL has shown that this type of source is more reliable with a longer lifetime (on the order of 6 to 9 months) due to better power efficiency. With a similar duty factor to BNL, we expect to have a comparable lifetime between source changes. The new source design reliably produces 90mA of H- beam current at 15Hz rep-rate, 250 mu s pulse width, and a duty factor of 0.38%.. The measured emittances at the end of the LEBT are horizontally epsilon(H) = 0.21(pi) mm(*) mrad and vertically epsilon(V) = 0.17(pi) mm(*) mrad. With 35kV extraction the power efficiency is 60mA/kW. The source design, along with data from a test stand and the LEBT, will be presented in this paper. C1 Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. RP Bollinger, DS (reprint author), Fermilab Natl Accelerator Lab, Box 500,MS 307, Batavia, IL 60510 USA. NR 4 TC 0 Z9 0 U1 0 U2 0 PU AMER INST PHYSICS PI MELVILLE PA 2 HUNTINGTON QUADRANGLE, STE 1NO1, MELVILLE, NY 11747-4501 USA SN 0094-243X BN 978-0-7354-1136-4 J9 AIP CONF PROC PY 2013 VL 1515 BP 312 EP 320 DI 10.1063/1.4792799 PG 9 WC Physics, Applied; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Physics GA BEK03 UT WOS:000317013500036 ER PT S AU Welton, RF Dudnikov, VG Han, BX Murray, SN Pennisi, TR Roseberry, RT Santana, M Stockli, MP AF Welton, R. F. Dudnikov, V. G. Han, B. X. Murray, S. N. Pennisi, T. R. Roseberry, R. T. Santana, M. Stockli, M. P. BE Tarvainen, O Kalvas, T TI Developing Reliable Internal Antennas and Standardizing Performance of H- RF Ion Sources SO THIRD INTERNATIONAL SYMPOSIUM ON NEGATIVE IONS, BEAMS AND SOURCES (NIBS 2012) SE AIP Conference Proceedings LA English DT Proceedings Paper CT 3rd International Symposium on Negative Ions, Beams and Sources (NIBS) CY SEP 03-07, 2012 CL Jyvaskyla, FINLAND SP Dehnel - Particle Accelerator Components & Engn Inc, Federat Finnish Learned Soc, Univ Jyvaskyla, Dept Phys, Univ Jyvaskyla DE negative ion sources; particle accelerators; ion formation AB The Spallation Neutron Source (SNS) now routinely operates near 1 MW of beam power on target with 30-40 mA peak current in the linac and an overall availability of similar to 90%. H- beam pulses (similar to 1 ms, 60Hz) are produced by a RF-driven, Cs-enhanced, multi-cusp ion source closely coupled to an electrostatic Low Energy Beam Transport (LEBT) which focuses the beam into an RFQ accelerator. The ion source and LEBT normally have a combined availability of similar to 99%. The source plasma is generated by RF excitation (2MHz, similar to 60kW) of a copper antenna which has been encased with a thickness of similar to 0.7 mm of porcelain enamel and is immersed into the plasma chamber. Failure of this coating material during operations has been a long-standing problem and a cause of downtime. This report describes new antenna installation criteria which have led to trouble free antenna performance over this last year, a significant improvement over previous years. These results suggest that inclusions and defects in the antenna coating play an important role in the failure process. This report also addresses the problem of inconsistent performance among our inventory of five ostensibly identical baseline SNS ion sources. Over the last several years only source #3 has regularly provided the required beam current to the SNS by outperforming the others by 5-10 mA. To address this, all baseline sources have been characterized on the ion source test stand and small physical differences between source #3 and the others have been identified and the impact of those differences on beam production assessed. C1 [Welton, R. F.; Han, B. X.; Murray, S. N.; Pennisi, T. R.; Roseberry, R. T.; Santana, M.; Stockli, M. P.] Oak Ridge Natl Lab, Spallat Neutron Source, POB 2008, Oak Ridge, TN 37830 USA. [Dudnikov, V. G.] Muons Inc, Batavia, IL 60510 USA. RP Welton, RF (reprint author), Oak Ridge Natl Lab, Spallat Neutron Source, POB 2008, Oak Ridge, TN 37830 USA. FU U.S. Department of Energy [DE-AC05-00OR22725] FX This work was performed at Oak Ridge National Laboratory, which is managed by UT-Battelle, LLC, under contract DE-AC05-00OR22725 for the U.S. Department of Energy. NR 6 TC 6 Z9 6 U1 0 U2 5 PU AMER INST PHYSICS PI MELVILLE PA 2 HUNTINGTON QUADRANGLE, STE 1NO1, MELVILLE, NY 11747-4501 USA SN 0094-243X BN 978-0-7354-1136-4 J9 AIP CONF PROC PY 2013 VL 1515 BP 341 EP 348 DI 10.1063/1.4792802 PG 8 WC Physics, Applied; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Physics GA BEK03 UT WOS:000317013500039 ER PT S AU Han, BX Stockli, MP Welton, RF Murray, SN Pennisi, TR Santana, M AF Han, B. X. Stockli, M. P. Welton, R. F. Murray, S. N., Jr. Pennisi, T. R. Santana, M. BE Tarvainen, O Kalvas, T TI Emittance Characterization of the Spallation Neutron Source H- Injector SO THIRD INTERNATIONAL SYMPOSIUM ON NEGATIVE IONS, BEAMS AND SOURCES (NIBS 2012) SE AIP Conference Proceedings LA English DT Proceedings Paper CT 3rd International Symposium on Negative Ions, Beams and Sources (NIBS) CY SEP 03-07, 2012 CL Jyvaskyla, FINLAND SP Dehnel - Particle Accelerator Components & Engn Inc, Federat Finnish Learned Societies, Univ Jyvaskyla, Dept Phys, Univ Jyvaskyla DE H- ion source; Low-energy beam transport; Beam emittance AB The H- injector for the Spallation Neutron Source (SNS) at Oak Ridge National Laboratory consists of a RF H- ion source and a compact electrostatic low-energy beam transport (LEBT) section. Up to 5 ion sources and up to 4 LEBT assemblies are alternated for the SNS beam operations. The beam current and emittance of the H- beam exiting the LEBT were characterized on the test-stand for different sources and LEBT assemblies in order to understand and minimize their performance variations. C1 [Han, B. X.; Stockli, M. P.; Welton, R. F.; Murray, S. N., Jr.; Pennisi, T. R.; Santana, M.] Oak Ridge Natl Lab, Spallat Neutron Source, Oak Ridge, TN 37831 USA. RP Han, BX (reprint author), Oak Ridge Natl Lab, Spallat Neutron Source, Oak Ridge, TN 37831 USA. NR 5 TC 1 Z9 1 U1 0 U2 2 PU AMER INST PHYSICS PI MELVILLE PA 2 HUNTINGTON QUADRANGLE, STE 1NO1, MELVILLE, NY 11747-4501 USA SN 0094-243X BN 978-0-7354-1136-4 J9 AIP CONF PROC PY 2013 VL 1515 BP 473 EP 480 DI 10.1063/1.4792818 PG 8 WC Physics, Applied; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Physics GA BEK03 UT WOS:000317013500055 ER PT S AU Stockli, MP Faircloth, D Kraus, W Ando, A Bollinger, DS Briefi, S Fantz, U Friedl, R Kashiwagi, M King, D Koivisto, H Han, BX Lettry, J Takeiri, Y Tarvainen, O Tsumori, K Welton, RF Wimmer, C AF Stockli, M. P. Faircloth, D. Kraus, W. Ando, A. Bollinger, D. S. Briefi, S. Fantz, U. Friedl, R. Kashiwagi, M. King, D. Koivisto, H. Han, B. X. Lettry, J. Takeiri, Y. Tarvainen, O. Tsumori, K. Welton, R. F. Wimmer, Ch BE Tarvainen, O Kalvas, T TI Workshop on Performance Variations in H- Ion Sources 2012: PV H(-)12 SO THIRD INTERNATIONAL SYMPOSIUM ON NEGATIVE IONS, BEAMS AND SOURCES (NIBS 2012) SE AIP Conference Proceedings LA English DT Proceedings Paper CT 3rd International Symposium on Negative Ions, Beams and Sources (NIBS) CY SEP 03-07, 2012 CL Jyvaskyla, FINLAND SP Dehnel - Particle Accelerator Components & Engn Inc, Federat Finnish Learned Soc, Univ Jyvaskyla, Dept Phys, Univ Jyvaskyla DE Cesium; H- ions; ion source AB This paper briefly summarizes a workshop held in Jyvaskyla the day after NIBS' 12. The half-day workshop aimed at globally capturing the issue of performance variations in H- sources. There was a focus on production facilities and facilities that work under production-like conditions, because there are often high expectations to be met. C1 [Stockli, M. P.; Han, B. X.; Wimmer, Ch] Oak Ridge Natl Lab, Spallat Neutron Source, Oak Ridge, TN 37831 USA. [Faircloth, D.] STFC, Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Kraus, W.; Briefi, S.; Fantz, U.; Friedl, R.; Wimmer, Ch] Max Planck Inst Plasma Phys, D-85748 Garching, Germany. [Ando, A.] Tohoku Univ, Grad Sch Engn, Sendai, Miyagi 980, Japan. [Bollinger, D. S.] Fermilab Natl Accelerator Lab, Batavia, IL 60543 USA. [Kashiwagi, M.] JAEA, Naka, Ibaraki 3110193, Japan. [King, D.] EURATOM CCFE Assoc, Culham Sci Ctr, Abingdon OX14 3DB, Oxon, England. [Koivisto, H.; Tarvainen, O.] Univ Jyvaskyla, Dept Phys, Jyvaskyla 40500, Finland. [Lettry, J.] CERN, Geneva, Switzerland. [Takeiri, Y.; Tsumori, K.] Natl Inst Fus Sci, Toki, Gifu 5095292, Japan. RP Stockli, MP (reprint author), Oak Ridge Natl Lab, Spallat Neutron Source, Oak Ridge, TN 37831 USA. NR 3 TC 0 Z9 0 U1 0 U2 2 PU AMER INST PHYSICS PI MELVILLE PA 2 HUNTINGTON QUADRANGLE, STE 1NO1, MELVILLE, NY 11747-4501 USA SN 0094-243X BN 978-0-7354-1136-4 J9 AIP CONF PROC PY 2013 VL 1515 BP 594 EP 597 DI 10.1063/1.4792832 PG 4 WC Physics, Applied; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Physics GA BEK03 UT WOS:000317013500069 ER PT J AU Abreu, P Aglietta, M Ahlers, M Ahn, EJ Albuquerque, IFM Allard, D Allekotte, I Allen, J Allison, P Almela, A Castillo, JA Alvarez-Muniz, J Batista, RA Ambrosio, M Aminaei, A Anchordoqui, L Andringa, S Anticic, T Aramo, C Arganda, E Arqueros, F Asorey, H Assis, P Aublin, J Ave, M Avenier, M Avila, G Backer, T Badescu, AM Balzer, M Barber, KB Barbosa, AF Bardenet, R Barroso, SLC Baughman, B Bauml, J Beatty, JJ Becker, BR Becker, KH Belletoile, A Bellido, JA BenZvi, S Berat, C Bertou, X Biermann, PL Billoir, P Blanco, F Blanco, M Bleve, C Blumer, H Bohacova, M Boncioli, D Bonifazi, C Bonino, R Borodai, N Brack, J Brancus, I Brogueira, P Brown, WC Bruijn, R Buchholz, P Bueno, A Burton, RE Caballero-Mora, KS Caccianiga, B Caramete, L Caruso, R Castellina, A Catalano, O Cataldi, G Cazon, L Cester, R Chauvin, J Cheng, SH Chiavassa, A Chinellato, JA Diaz, JC Chudoba, J Cilmo, M Clay, RW Coluccia, MR Conceicao, R Contreras, F Cook, H Cooper, MJ Coppens, J Cordier, A Coutu, S Covault, CE Creusot, A Criss, A Cronin, J Curutiu, A Dagoret-Campagne, S Dallier, R Daniel, B Dasso, S Daumiller, K Dawson, BR de Almeida, RM De Domenico, M De Donato, C de Jong, SJ De La Vega, G de Mello, WJM Neto, JRTD De Mitri, I de Souza, V de Vries, KD del Peral, L del Rio, M Deligny, O Dembinski, H Dhital, N Di Giulio, C Castro, MLD Diep, PN Diogo, F Dobrigkeit, C Docters, W D'Olivo, JC Dong, PN Dorofeev, A dos Anjos, JC Dova, MT D'Urso, D Dutan, I Ebr, J Engel, R Erdmann, M Escobar, CO Espadanal, J Etchegoyen, A San Luis, PF Falcke, H Farrar, G Fauth, AC Fazzini, N Ferguson, AP Fick, B Filevich, A Filipcic, A Fliescher, S Fracchiolla, CE Fraenkel, ED Fratu, O Frohlich, U Fuchs, B Gaior, R Gamarra, RF Gambetta, S Garcia, B Roca, STG Garcia-Gamez, D Garcia-Pinto, D Bravo, AG Gemmeke, H Ghia, PL Giller, M Gitto, J Glass, H Gold, MS Golup, G Albarracin, FG Berisso, MG Vitale, PFG Goncalves, P Gonzalez, JG Gookin, B Gorgi, A Gouffon, P Grashorn, E Grebe, S Griffith, N Grigat, M Grillo, AF Guardincerri, Y Guarino, F Guedes, GP Hansen, P Harari, D Harrison, TA Harton, JL Haungs, A Hebbeker, T Heck, D Herve, AE Hojvat, C Hollon, N Holmes, VC Homola, P Horandel, JR Horvath, P Hrabovsky, M Huber, D Huege, T Insolia, A Ionita, F Italiano, A Jarne, C Jiraskova, S Josebachuili, M Kadija, K Kampert, KH Karhan, P Kasper, P Katkov, I Kegl, B Keilhauer, B Keivani, A Kelley, JL Kemp, E Kieckhafer, RM Klages, HO Kleifges, M Kleinfeller, J Knapp, J Koang, DH Kotera, K Krohm, N Kromer, O Kruppke-Hansen, D Kuehn, F Kuempel, D Kulbartz, JK Kunka, N La Rosa, G Lachaud, C LaHurd, D Latronico, L Lauer, R Lautridou, P Le Coz, S Leao, MSAB Lebrun, D Lebrun, P de Oliveira, MAL Letessier-Selvon, A Lhenry-Yvon, I Link, K Lopez, R Aguera, AL Louedec, K Bahilo, JL Lu, L Lucero, A Ludwig, M Lyberis, H Maccarone, MC Macolino, C Maldera, S Mandat, D Mantsch, P Mariazzi, AG Marin, J Marin, V Maris, IC Falcon, HRM Marsella, G Martello, D Martin, L Martinez, H Bravo, OM Mathes, HJ Matthews, J Matthews, JAJ Matthiae, G Maurel, D Maurizio, D Mazur, PO Medina-Tanco, G Melissas, M Melo, D Menichetti, E Menshikov, A Mertsch, P Meurer, C Micanovic, S Micheletti, MI Minaya, IA Miramonti, L Molina-Bueno, L Mollerach, S Monasor, M Ragaigne, DM Montanet, F Morales, B Morello, C Moreno, E Moreno, JC Mostafa, M Moura, CA Muller, MA Muller, G Munchmeyer, M Mussa, R Navarra, G Navarro, JL Navas, S Necesal, P Nellen, L Nelles, A Neuser, J Nhung, PT Niechciol, M Niemietz, L Nierstenhoefer, N Nitz, D Nosek, D Nozka, L Oehlschlager, J Olinto, A Ortiz, M Pacheco, N Selmi-Dei, DP Palatka, M Pallotta, J Palmieri, N Parente, G Parizot, E Parra, A Pastor, S Paul, T Pech, M Pekala, J Pelayo, R Pepe, IM Perrone, L Pesce, R Petermann, E Petrera, S Petrolini, A Petrov, Y Pfendner, C Piegaia, R Pierog, T Pieroni, P Pimenta, M Pirronello, V Platino, M Plum, M Ponce, VH Pontz, M Porcelli, A Privitera, P Prouza, M Quel, EJ Querchfeld, S Rautenberg, J Ravel, O Ravignani, D Revenu, B Ridky, J Riggi, S Risse, M Ristori, P Rivera, H Rizi, V Roberts, J de Carvalho, WR Rodriguez, G Cabo, IR Martino, JR Rojo, JR Rodriguez-Frias, MD Ros, G Rosado, J Rossler, T Roth, M Rouille-d'Orfeuil, B Roulet, E Rovero, AC Ruehle, C Saftoiu, A Salamida, F Salazar, H Greus, FS Salina, G Sanchez, F Santo, CE Santos, E Santos, EM Sarazin, F Sarkar, B Sarkar, S Sato, R Scharf, N Scherini, V Schieler, H Schiffer, P Schmidt, A Scholten, O Schoorlemmer, H Schovancova, J Schovanek, P Schroder, F Schulte, S Schuster, D Sciutto, SJ Scuderi, M Segreto, A Settimo, M Shadkam, A Shellard, RC Sidelnik, I Sigl, G Sima, O Smialkowski, A Smida, R Snow, GR Sommers, P Sorokin, J Spinka, H Squartini, R Srivastava, YN Stanic, S Stapleton, J Stasielak, J Stephan, M Stutz, A Suarez, F Suomijarvi, T Supanitsky, AD Susa, T Sutherland, MS Swain, J Szadkowski, Z Szuba, M Tapia, A Tartare, M Tascau, O Tcaciuc, R Thao, NT Thomas, D Tiffenberg, J Timmermans, C Tkaczyk, W Peixoto, CJT Toma, G Tomankova, L Tome, B Tonachini, A Travnicek, P Tridapalli, DB Tristram, G Trovato, E Tueros, M Ulrich, R Unger, M Urban, M Galicia, JFV Valino, I Valore, L van den Berg, AM Varela, E Cardenas, BV Vazquez, JR Vazquez, RA Veberic, D Verzi, V Vicha, J Videla, M Villasenor, L Wahlberg, H Wahrlich, P Wainberg, O Walz, D Watson, AA Weber, M Weidenhaupt, K Weindl, A Werner, F Westerhoff, S Whelan, BJ Widom, A Wieczorek, G Wiencke, L Wilczynska, B Wilczynski, H Will, M Williams, C Winchen, T Wommer, M Wundheiler, B Yamamoto, T Yapici, T Younk, P Yuan, G Yushkov, A Garcia, BZ Zas, E Zavrtanik, D Zavrtanik, M Zaw, I Zepeda, A Zhu, Y Silva, MZ Ziolkowski, M AF Abreu, P. 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Santo, C. E. Santos, E. Santos, E. M. Sarazin, F. Sarkar, B. Sarkar, S. Sato, R. Scharf, N. Scherini, V. Schieler, H. Schiffer, P. Schmidt, A. Scholten, O. Schoorlemmer, H. Schovancova, J. Schovanek, P. Schroeder, F. Schulte, S. Schuster, D. Sciutto, S. J. Scuderi, M. Segreto, A. Settimo, M. Shadkam, A. Shellard, R. C. Sidelnik, I. Sigl, G. Sima, O. Smialkowski, A. Smida, R. Snow, G. R. Sommers, P. Sorokin, J. Spinka, H. Squartini, R. Srivastava, Y. N. Stanic, S. Stapleton, J. Stasielak, J. Stephan, M. Stutz, A. Suarez, F. Suomijaervi, T. Supanitsky, A. D. Susa, T. Sutherland, M. S. Swain, J. Szadkowski, Z. Szuba, M. Tapia, A. Tartare, M. Tascau, O. Tcaciuc, R. Thao, N. T. Thomas, D. Tiffenberg, J. Timmermans, C. Tkaczyk, W. Todero Peixoto, C. J. Toma, G. Tomankova, L. Tome, B. Tonachini, A. Travnicek, P. Tridapalli, D. B. Tristram, G. Trovato, E. Tueros, M. Ulrich, R. Unger, M. Urban, M. Valdes Galicia, J. F. Valino, I. Valore, L. van den Berg, A. M. Varela, E. Vargas Cardenas, B. Vazquez, J. R. Vazquez, R. A. Veberic, D. Verzi, V. Vicha, J. Videla, M. Villasenor, L. Wahlberg, H. Wahrlich, P. Wainberg, O. Walz, D. Watson, A. A. Weber, M. Weidenhaupt, K. Weindl, A. Werner, F. Westerhoff, S. Whelan, B. J. Widom, A. Wieczorek, G. Wiencke, L. Wilczynska, B. Wilczynski, H. Will, M. Williams, C. Winchen, T. Wommer, M. Wundheiler, B. Yamamoto, T. Yapici, T. Younk, P. Yuan, G. Yushkov, A. Zamorano Garcia, B. Zas, E. Zavrtanik, D. Zavrtanik, M. Zaw, I. Zepeda, A. Zhu, Y. Zimbres Silva, M. Ziolkowski, M. CA Pierre Auger Collaboration TI Ultrahigh Energy Neutrinos at the Pierre Auger Observatory SO ADVANCES IN HIGH ENERGY PHYSICS LA English DT Review ID COSMIC-RAYS; AIR-SHOWERS; TAU-NEUTRINOS; FLUX; SPECTRUM; SEARCH; ARRAY; LIMIT AB The observation of ultrahigh energy neutrinos (UHE nu s) has become a priority in experimental astroparticle physics. UHE nu s can be detected with a variety of techniques. In particular, neutrinos can interact in the atmosphere (downward-going nu) or in the Earth crust (Earth-skimming nu), producing air showers that can be observed with arrays of detectors at the ground. With the surface detector array of the Pierre Auger Observatory we can detect these types of cascades. The distinguishing signature for neutrino events is the presence of very inclined showers produced close to the ground (i.e., after having traversed a large amount of atmosphere). In this work we review the procedure and criteria established to search for UHE nu s in the data collected with the ground array of the Pierre Auger Observatory. This includes Earth-skimming as well as downward-going neutrinos. No neutrino candidates have been found, which allows us to place competitive limits to the diffuse flux of UHE nu s in the EeV range and above. 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[Caccianiga, B.; Miramonti, L.; Rivera, H.; Scherini, V.] Sezione Ist Nazl Fis Nucl, Milan, Italy. [Caruso, R.; De Domenico, M.; Insolia, A.; Italiano, A.; Pirronello, V.; Scuderi, M.; Trovato, E.] Univ Catania, Catania, Italy. [Caruso, R.; De Domenico, M.; Insolia, A.; Italiano, A.; Pirronello, V.; Scuderi, M.; Trovato, E.] Sezione Ist Nazl Fis Nucl, Catania, Italy. [Catalano, O.; La Rosa, G.; Maccarone, M. C.; Segreto, A.] Ist Astrofis Spaziale & Fis Cosm Palermo INAF, Palermo, Italy. [Cataldi, G.; Coluccia, M. R.; De Mitri, I.; Martello, D.] Univ Salento, Dipartimento Fis, Lecce, Italy. [Cataldi, G.; Coluccia, M. R.; De Mitri, I.; Marsella, G.; Martello, D.; Perrone, L.] Sezione Ist Nazl Fis Nucl, Lecce, Italy. [Cester, R.; Maurizio, D.; Menichetti, E.; Mussa, R.; Tonachini, A.] Univ Turin, Turin, Italy. [Diaz, J. Chirinos; Dhital, N.; Fick, B.; Kieckhafer, R. M.; Nitz, D.; Yapici, T.] Michigan Technol Univ, Houghton, MI 49931 USA. [Coppens, J.; de Jong, S. J.; Grebe, S.; Nelles, A.; Schoorlemmer, H.; Timmermans, C.] Nikhef, Amsterdam, Netherlands. [Cronin, J.; San Luis, P. Facal; Hollon, N.; Ionita, F.; Kotera, K.; Monasor, M.; Olinto, A.; Privitera, P.; Rouille-d'Orfeuil, B.; Williams, C.; Yamamoto, T.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Dasso, S.; Rovero, A. C.; Supanitsky, A. D.] Inst Astron & Fis Espacio CONICET UBA, Buenos Aires, DF, Argentina. [Dasso, S.; Guardincerri, Y.; Piegaia, R.; Pieroni, P.; Tiffenberg, J.] Univ Buenos Aires, FCEyN, Dept Fis, Buenos Aires, DF, Argentina. [Dasso, S.; Guardincerri, Y.; Piegaia, R.; Pieroni, P.; Tiffenberg, J.] Consejo Nacl Invest Cient & Tecn, RA-1033 Buenos Aires, DF, Argentina. [de Almeida, R. M.] Univ Fed Fluminense, EEIMVR, Volta Redonda, RJ, Brazil. [De La Vega, G.; Garcia, B.; Gitto, J.; Videla, M.] Natl Technol Univ, Fac Mendoza CONICET CNEA, Mendoza, Argentina. [de Souza, V.; Todero Peixoto, C. J.] Univ Sao Paulo, Inst Fis, Sao Carlos, SP, Brazil. [de Vries, K. D.; Docters, W.; Fraenkel, E. D.; Scholten, O.; van den Berg, A. M.] Univ Groningen, Kernfys Versneller Inst, Groningen, Netherlands. [Deligny, O.; Dong, P. N.; Lhenry-Yvon, I.; Lyberis, H.; Salamida, F.; Suomijaervi, T.] Univ Paris 11, IPNO, CNRS IN2P3, Orsay, France. [Di Giulio, C.; Petrera, S.; Rizi, V.] Univ Aquila, I-67100 Laquila, Italy. [Di Giulio, C.; Petrera, S.; Rizi, V.] Ist Nazl Fis Nucl, Laquila, Italy. [Diep, P. N.; Dong, P. N.; Nhung, P. T.; Thao, N. T.] INST, Hanoi, Vietnam. [Erdmann, M.; Fliescher, S.; Grigat, M.; Hebbeker, T.; Kuempel, D.; Meurer, C.; Mueller, G.; Plum, M.; Scharf, N.; Schiffer, P.; Schulte, S.; Stephan, M.; Walz, D.; Weidenhaupt, K.; Winchen, T.] Rhein Westfal TH Aachen, Phy Inst A 3, Aachen, Germany. [Falcke, H.] ASTRON, Dwingeloo, Netherlands. [Filipcic, A.; Szadkowski, Z.; Veberic, D.; Zavrtanik, D.; Zavrtanik, M.] Jozef Stefan Inst, Ljubljana, Slovenia. [Filipcic, A.; Stanic, S.; Veberic, D.; Zavrtanik, D.; Zavrtanik, M.] Univ Nova Gorica, Lab Astroparticle Phys, Nova Gorica, Slovenia. [Gambetta, S.; Pesce, R.; Petrolini, A.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Gambetta, S.; Pesce, R.; Petrolini, A.] Ist Nazl Fis Nucl, I-16146 Genoa, Italy. [Giller, M.; Smialkowski, A.; Tkaczyk, W.; Wieczorek, G.] Univ Lodz, PL-90131 Lodz, Poland. [Grillo, A. F.] Ist Nazl Fis Nucl, Lab Nazl Gran Sasso, Laquila, Italy. [Guedes, G. P.] Univ Estadual Feira de Santana, Feira De Santana, Brazil. [Horvath, P.; Hrabovsky, M.; Rossler, T.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Karhan, P.; Nosek, D.] Charles Univ Prague, Fac Math & Phys, Inst Particle & Nucl Phys, Prague, Czech Republic. [Keivani, A.; Matthews, J.; Shadkam, A.; Sutherland, M. S.; Yuan, G.] Louisiana State Univ, Baton Rouge, LA 70803 USA. [Kulbartz, J. K.; Schiffer, P.; Sigl, G.] Univ Hamburg, Hamburg, Germany. [Leao, M. S. A. B.; Leigui de Oliveira, M. A.; Moura, C. A.] Univ Fed ABC, Santo Andre, SP, Brazil. [Lopez, R.; Martinez Bravo, O.; Moreno, E.; Pelayo, R.; Salazar, H.; Varela, E.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Marquez Falcon, H. R.; Villasenor, L.] Univ Michoacana, Morelia, Michoacan, Mexico. [Marsella, G.; Perrone, L.] Univ Salento, Dipartimento Ingn Innovaz, Lecce, Italy. [Martinez, H.; Zepeda, A.] IPN CINVESTAV, Ctr Invest & Estudios Avanzados, Mexico City, DF, Mexico. [Matthews, J.] Southern Univ, Baton Rouge, LA USA. [Mertsch, P.; Sarkar, S.] Univ Oxford, Rudolf Peierls Ctr Theoret Phys, Oxford, England. [Micheletti, M. I.] CONICET UNR, Inst Fis Rosario IFIR, Rosario, Santa Fe, Argentina. [Micheletti, M. I.] Fac Ciencias Bioquim & Farmaceut UNR, Rosario, Santa Fe, Argentina. [Pallotta, J.; Quel, E. J.; Ristori, P.] CITEDEF, Ctr Invest Laseres & Aplicac, San Carlos De Bariloche, Rio Negro, Argentina. [Pallotta, J.; Quel, E. J.; Ristori, P.] Consejo Nacl Invest Cient & Tecn, San Carlos De Bariloche, Rio Negro, Argentina. [Pastor, S.] Univ Valencia, CSIC, Inst Fis Corpuscular, Valencia, Spain. [Paul, T.; Srivastava, Y. N.; Swain, J.; Widom, A.] Northeastern Univ, Boston, MA 02115 USA. [Pepe, I. M.] Univ Fed Bahia, Salvador, BA, Brazil. [Petermann, E.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Sarazin, F.; Schuster, D.; Wiencke, L.] Colorado Sch Mines, Golden, CO 80401 USA. [Sima, O.] Univ Bucharest, Dept Phys, Bucharest, Romania. [Spinka, H.] Argonne Natl Lab, Argonne, IL 60439 USA. [Yamamoto, T.] Konan Univ, Kobe, Hyogo, Japan. [Younk, P.] Los Alamos Natl Lab, Los Alamos, NM USA. [Zaw, I.] NYU Abu Dhabi, Abu Dhabi, U Arab Emirates. RP Abreu, P (reprint author), Univ Tecn Lisboa, LIP, Lisbon, Portugal. RI Todero Peixoto, Carlos Jose/G-3873-2012; Nosek, Dalibor/F-1129-2017; Navas, Sergio/N-4649-2014; Blanco, Francisco/F-1131-2015; Sao Carlos Institute of Physics, IFSC/USP/M-2664-2016; Conceicao, Ruben/L-2971-2014; Beatty, James/D-9310-2011; Guarino, Fausto/I-3166-2012; Bonino, Raffaella/S-2367-2016; Rodriguez Frias, Maria /A-7608-2015; Inst. of Physics, Gleb Wataghin/A-9780-2017; De Mitri, Ivan/C-1728-2017; Falcke, Heino/H-5262-2012; Insolia, Antonio/M-3447-2015; Petrolini, Alessandro/H-3782-2011; de Mello Neto, Joao/C-5822-2013; Lozano-Bahilo, Julio/F-4881-2016; scuderi, mario/O-7019-2014; zas, enrique/I-5556-2015; Arqueros, Fernando/K-9460-2014; Moura Santos, Edivaldo/K-5313-2016; Gouffon, Philippe/I-4549-2012; de Almeida, Rogerio/L-4584-2016; De Domenico, Manlio/B-5826-2014; Abreu, Pedro/L-2220-2014; Dutan, Ioana/C-2337-2011; Sima, Octavian/C-3565-2011; Di Giulio, Claudio/B-3319-2015; Bueno, Antonio/F-3875-2015; Albuquerque, Ivone/H-4645-2012; Parente, Gonzalo/G-8264-2015; Alvarez-Muniz, Jaime/H-1857-2015; Valino, Ines/J-8324-2012; Carvalho Jr., Washington/H-9855-2015; Espadanal, Joao/I-6618-2015; De Donato, Cinzia/J-9132-2015; Martello, Daniele/J-3131-2012; Ridky, Jan/H-6184-2014; Chudoba, Jiri/G-7737-2014; Horvath, Pavel/G-6334-2014; Garcia Pinto, Diego/J-6724-2014; Pastor, Sergio/J-6902-2014; Rosado, Jaime/K-9109-2014; Espirito Santo, Maria Catarina/L-2341-2014; Pimenta, Mario/M-1741-2013; Ros, German/L-4764-2014; Brogueira, Pedro/K-3868-2012; Alves Batista, Rafael/K-6642-2012; Moura, Celio/K-5672-2013; dos Santos, Eva/N-6351-2013; de souza, Vitor/D-1381-2012; Prouza, Michael/F-8514-2014; Mandat, Dusan/G-5580-2014; Pech, Miroslav/G-5760-2014; Bohacova, Martina/G-5898-2014; Cazon, Lorenzo/G-6921-2014; Schovanek, Petr/G-7117-2014; Vicha, Jakub/G-8440-2014; Travnicek, Petr/G-8814-2014; Smida, Radomir/G-6314-2014; Goncalves, Patricia /D-8229-2013; Assis, Pedro/D-9062-2013; Sarkar, Subir/G-5978-2011; Tome, Bernardo/J-4410-2013; Caramete, Laurentiu/C-2328-2011; Nierstenhofer, Nils/H-3699-2013; Pakk Selmi-Dei, Daniel/H-2675-2013; Ebr, Jan/H-8319-2012; Badescu, Alina/B-6087-2012; Chinellato, Carola Dobrigkeit /F-2540-2011; Fauth, Anderson/F-9570-2012 OI Del Peral, Luis/0000-0003-2580-5668; Coutu, Stephane/0000-0003-2923-2246; Dembinski, Hans/0000-0003-3337-3850; Catalano, Osvaldo/0000-0002-9554-4128; Ravignani, Diego/0000-0001-7410-8522; Kothandan, Divay/0000-0001-9048-7518; La Rosa, Giovanni/0000-0002-3931-2269; Mussa, Roberto/0000-0002-0294-9071; Ulrich, Ralf/0000-0002-2535-402X; Garcia, Beatriz/0000-0003-0919-2734; Rodriguez Fernandez, Gonzalo/0000-0002-4683-230X; Zamorano, Bruno/0000-0002-4286-2835; Bonino, Raffaella/0000-0002-4264-1215; Knapp, Johannes/0000-0003-1519-1383; Todero Peixoto, Carlos Jose/0000-0003-3669-8212; Marsella, Giovanni/0000-0002-3152-8874; Asorey, Hernan/0000-0002-4559-8785; Rizi, Vincenzo/0000-0002-5277-6527; Petrera, Sergio/0000-0002-6029-1255; Andringa, Sofia/0000-0002-6397-9207; Aramo, Carla/0000-0002-8412-3846; Aglietta, Marco/0000-0001-8354-5388; Maccarone, Maria Concetta/0000-0001-8722-0361; Castellina, Antonella/0000-0002-0045-2467; maldera, simone/0000-0002-0698-4421; Matthews, James/0000-0002-1832-4420; Yuan, Guofeng/0000-0002-1907-8815; Mertsch, Philipp/0000-0002-2197-3421; Nosek, Dalibor/0000-0001-6219-200X; de Jong, Sijbrand/0000-0002-3120-3367; Sigl, Guenter/0000-0002-4396-645X; Cataldi, Gabriella/0000-0001-8066-7718; Navarro Quirante, Jose Luis/0000-0002-9915-1735; Mantsch, Paul/0000-0002-8382-7745; Salamida, Francesco/0000-0002-9306-8447; Segreto, Alberto/0000-0001-7341-6603; Navas, Sergio/0000-0003-1688-5758; Blanco, Francisco/0000-0003-4332-434X; Conceicao, Ruben/0000-0003-4945-5340; Beatty, James/0000-0003-0481-4952; Guarino, Fausto/0000-0003-1427-9885; Rodriguez Frias, Maria /0000-0002-2550-4462; De Mitri, Ivan/0000-0002-8665-1730; Falcke, Heino/0000-0002-2526-6724; Insolia, Antonio/0000-0002-9040-1566; Petrolini, Alessandro/0000-0003-0222-7594; de Mello Neto, Joao/0000-0002-3234-6634; Lozano-Bahilo, Julio/0000-0003-0613-140X; scuderi, mario/0000-0001-9026-5317; zas, enrique/0000-0002-4430-8117; Arqueros, Fernando/0000-0002-4930-9282; Moura Santos, Edivaldo/0000-0002-2818-8813; Gouffon, Philippe/0000-0001-7511-4115; de Almeida, Rogerio/0000-0003-3104-2724; De Domenico, Manlio/0000-0001-5158-8594; Abreu, Pedro/0000-0002-9973-7314; Di Giulio, Claudio/0000-0002-0597-4547; Bueno, Antonio/0000-0002-7439-4247; Albuquerque, Ivone/0000-0001-7328-0136; Parente, Gonzalo/0000-0003-2847-0461; Alvarez-Muniz, Jaime/0000-0002-2367-0803; Valino, Ines/0000-0001-7823-0154; Carvalho Jr., Washington/0000-0002-2328-7628; Espadanal, Joao/0000-0002-1301-8061; De Donato, Cinzia/0000-0002-9725-1281; Martello, Daniele/0000-0003-2046-3910; Ridky, Jan/0000-0001-6697-1393; Horvath, Pavel/0000-0002-6710-5339; Garcia Pinto, Diego/0000-0003-1348-6735; Rosado, Jaime/0000-0001-8208-9480; Espirito Santo, Maria Catarina/0000-0003-1286-7288; Pimenta, Mario/0000-0002-2590-0908; Ros, German/0000-0001-6623-1483; Brogueira, Pedro/0000-0001-6069-4073; Alves Batista, Rafael/0000-0003-2656-064X; Moura, Celio/0000-0001-7991-9025; dos Santos, Eva/0000-0002-0474-8863; Prouza, Michael/0000-0002-3238-9597; Cazon, Lorenzo/0000-0001-6748-8395; Goncalves, Patricia /0000-0003-2042-3759; Assis, Pedro/0000-0001-7765-3606; Sarkar, Subir/0000-0002-3542-858X; Tome, Bernardo/0000-0002-7564-8392; Ebr, Jan/0000-0001-8807-6162; Chinellato, Carola Dobrigkeit /0000-0002-1236-0789; Fauth, Anderson/0000-0001-7239-0288 FU Comision Nacional de Energia Atomica; Fundacion Antorchas; Gobierno De La Provincia de Mendoza; Municipalidad de Malargue; NDM Holdings; Valle Las Lenas; Australian Research Council; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq); Financiadora de Estudos e Projetos (FINEP); Fundacao de Amparo a Pesquisa do Estado de Rio de Janeiro (FAPERJ); Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); Ministerio de Ciencia e Tecnologia (MCT), Brazil; AVCR, Czech Republic [AV0Z10100502, AV0Z10100522, GAAV KJB100100904, MSMT-CR LA08016, LG11044, MEB111003, MSM0021620859, LA08015, TACR TA01010517]; Centre de Calcul IN2P3/CNRS; Centre National de la Recherche Scientifique (CNRS); Conseil Regional Ile-deFrance; Departement Physique Nucleaire et Corpusculaire [PNC-IN2P3/CNRS]; Departement Sciences de l'Univers (SDU-INSU/CNRS), France; Bundesministerium fur Bildung und Forschung (BMBF); Deutsche Forschungsgemeinschaft (DFG); Finanzministerium Baden-Wurttemberg; Helmholtz-Gemeinschaft Deutscher Forschungszentren (HGF); Ministerium fur Wissenschaft und Forschung; Nordrhein-Westfalen; Ministerium fur Wissenschaft; Forschung und Kunst; Baden-Wurttemberg, Germany FX The successful installation, commissioning, and operation of the Pierre Auger Observatory would not have been possible without the strong commitment and effort from the technical and administrative staff in Malargue. The authors are very grateful to the following agencies and organizations for financial support: Comision Nacional de Energia Atomica, Fundacion Antorchas, Gobierno De La Provincia de Mendoza, Municipalidad de Malargue, NDM Holdings and Valle Las Lenas, in gratitude for their continuing cooperation over land access, Argentina; the Australian Research Council; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq), Financiadora de Estudos e Projetos (FINEP), Fundacao de Amparo a Pesquisa do Estado de Rio de Janeiro (FAPERJ), Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP), Ministerio de Ciencia e Tecnologia (MCT), Brazil; AVCR AV0Z10100502 and AV0Z10100522, GAAV KJB100100904, MSMT-CR LA08016, LG11044, MEB111003, MSM0021620859, LA08015, and TACR TA01010517, Czech Republic; Centre de Calcul IN2P3/CNRS, Centre National de la Recherche Scientifique (CNRS), Conseil Regional Ile-deFrance, Departement Physique Nucleaire et Corpusculaire (PNC-IN2P3/CNRS), Departement Sciences de l'Univers (SDU-INSU/CNRS), France; Bundesministerium fur Bildung und Forschung (BMBF), Deutsche Forschungsgemeinschaft (DFG), Finanzministerium Baden-Wurttemberg, Helmholtz-Gemeinschaft Deutscher Forschungszentren (HGF), Ministerium fur Wissenschaft und Forschung, Nordrhein-Westfalen, Ministerium fur Wissenschaft, Forschung und Kunst, Baden-Wurttemberg, Germany; Istituto Nazionale di Fisica Nucleare (INFN), Ministero dell'Istruzione, dell'Universita e della Ricerca (MIUR), Italy; Consejo Nacional de Ciencia y Tecnologia (CONACYT), Mexico; Ministerie van Onderwijs, Cultuur en Wetenschap, Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Stichting voor Fundamenteel Onderzoek der Materie (FOM), The Netherlands; Ministry of Science and Higher Education, Grants no. N N202 200239 and N N202 2038, Poland; Fundacao para a Ciencia e a Tecnologia, Portugal; Ministry for Higher Education, Science, and Technology, Slovenian Research Agency, Slovenia; Comunidad de Madrid, Consejeria de Educacion de la Comunidad de Castilla La Mancha, FEDER funds, Ministerio de Ciencia e Innovacion and Consolider-Ingenio 2010 (CPAN), Xunta de Galicia, Spain; Science and Technology Facilities Council, UK; Department of Energy, Contract nos. DE-AC02-07CH11359 and DE-FR02-04ER41300, National Science Foundation, Grant no. 0450696, The Grainger Foundation, USA; NAFOSTED, Vietnam; ALFA-EC/HELEN and UNESCO. NR 50 TC 15 Z9 15 U1 3 U2 72 PU HINDAWI PUBLISHING CORPORATION PI NEW YORK PA 410 PARK AVENUE, 15TH FLOOR, #287 PMB, NEW YORK, NY 10022 USA SN 1687-7357 J9 ADV HIGH ENERGY PHYS JI Adv. High. Energy Phys. PY 2013 AR 708680 DI 10.1155/2013/708680 PG 18 WC Physics, Particles & Fields SC Physics GA 120WS UT WOS:000317204500001 ER PT J AU Samset, BH Myhre, G Schulz, M Balkanski, Y Bauer, S Berntsen, TK Bian, H Bellouin, N Diehl, T Easter, RC Ghan, SJ Iversen, T Kinne, S Kirkevag, A Lamarque, JF Lin, G Liu, X Penner, JE Seland, O Skeie, RB Stier, P Takemura, T Tsigaridis, K Zhang, K AF Samset, B. H. Myhre, G. Schulz, M. Balkanski, Y. Bauer, S. Berntsen, T. K. Bian, H. Bellouin, N. Diehl, T. Easter, R. C. Ghan, S. J. Iversen, T. Kinne, S. Kirkevag, A. Lamarque, J. -F. Lin, G. Liu, X. Penner, J. E. Seland, O. Skeie, R. B. Stier, P. Takemura, T. Tsigaridis, K. Zhang, K. TI Black carbon vertical profiles strongly affect its radiative forcing uncertainty SO ATMOSPHERIC CHEMISTRY AND PHYSICS LA English DT Article ID CLIMATE MODELS; AEROSOL DIRECT; AEROCOM; SIMULATIONS; SENSITIVITY; ATMOSPHERE; EMISSIONS; TRANSPORT; POLLUTION AB The impact of black carbon (BC) aerosols on the global radiation balance is not well constrained. Here twelve global aerosol models are used to show that at least 20% of the present uncertainty in modeled BC direct radiative forcing (RF) is due to diversity in the simulated vertical profile of BC mass. Results are from phases 1 and 2 of the global aerosol model intercomparison project (AeroCom). Additionally, a significant fraction of the variability is shown to come from high altitudes, as, globally, more than 40% of the total BC RF is exerted above 5 km. BC emission regions and areas with transported BC are found to have differing characteristics. These insights into the importance of the vertical profile of BC lead us to suggest that observational studies are needed to better characterize the global distribution of BC, including in the upper troposphere. C1 [Samset, B. H.; Myhre, G.; Berntsen, T. K.; Skeie, R. B.] CICERO, Oslo, Norway. [Schulz, M.; Iversen, T.; Kirkevag, A.; Seland, O.] Norwegian Meteorol Inst, Oslo, Norway. [Balkanski, Y.] UVSQ, CNRS, CEA, Lab Sci Climat & Environm, Gif Sur Yvette, France. [Bauer, S.; Tsigaridis, K.] NASA, Goddard Inst Space Studies, New York, NY 10025 USA. [Bauer, S.; Tsigaridis, K.] Columbia Earth Inst, New York, NY USA. [Bian, H.] Univ Maryland Baltimore Cty, Joint Ctr Earth Syst Technol, Baltimore, MD 21228 USA. [Bellouin, N.] Met Off, Hadley Ctr, Exeter, Devon, England. [Diehl, T.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Diehl, T.] Univ Space Res Assoc, Columbia, MD USA. [Easter, R. C.; Ghan, S. J.; Liu, X.; Zhang, K.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Kinne, S.; Zhang, K.] Max Planck Inst Meteorol, D-20146 Hamburg, Germany. [Iversen, T.] Univ Oslo, Dept Geosci, Oslo, MN USA. [Lamarque, J. -F.] Natl Ctr Atmospher Res, NCAR Earth Syst Lab, Boulder, CO 80307 USA. [Lin, G.; Penner, J. E.] Univ Michigan, Dept Atmospher Ocean & Space Sci, Ann Arbor, MI 48109 USA. [Stier, P.] Univ Oxford, Dept Phys, Oxford, England. [Takemura, T.] Kyushu Univ, Res Inst Appl Mech, Fukuoka 812, Japan. [Iversen, T.] ECMWF, Reading RG2 9AX, Berks, England. RP Samset, BH (reprint author), CICERO, Oslo, Norway. EM b.h.samset@cicero.uio.no RI Stier, Philip/B-2258-2008; Schulz, Michael/A-6930-2011; U-ID, Kyushu/C-5291-2016; Ghan, Steven/H-4301-2011; Takemura, Toshihiko/C-2822-2009; Penner, Joyce/J-1719-2012; Liu, Xiaohong/E-9304-2011; Balkanski, Yves/A-6616-2011; Lamarque, Jean-Francois/L-2313-2014; Bauer, Susanne/P-3082-2014; Kyushu, RIAM/F-4018-2015; Myhre, Gunnar/A-3598-2008; Skeie, Ragnhild/K-1173-2015; Zhang, Kai/F-8415-2010 OI Stier, Philip/0000-0002-1191-0128; Bellouin, Nicolas/0000-0003-2109-9559; Schulz, Michael/0000-0003-4493-4158; Ghan, Steven/0000-0001-8355-8699; Takemura, Toshihiko/0000-0002-2859-6067; Liu, Xiaohong/0000-0002-3994-5955; Balkanski, Yves/0000-0001-8241-2858; Lamarque, Jean-Francois/0000-0002-4225-5074; Myhre, Gunnar/0000-0002-4309-476X; Skeie, Ragnhild/0000-0003-1246-4446; Zhang, Kai/0000-0003-0457-6368 FU US Department of Energy, Office of Science, Scientific Discovery through Advanced Computing (SciDAC) Program; Office of Science Earth System Modeling Program; National Science Foundation; DOE by Battelle Memorial Institute [DE-AC06-76RLO 1830]; FP6 project EUCAARI [34684]; Research Council of Norway through the EarthClim [207711/E10]; NOTUR/NorStore projects; Norwegian Space Centre through PM-VRAE; EU; Research Council of Norway; NASA-MAP (NASA award) [NNX09AK32G]; Joint DECC/Defra Met Office Hadley Centre Climate Programme [GA01101] FX S. Ghan, X. Liu and R. Easter were funded by the US Department of Energy, Office of Science, Scientific Discovery through Advanced Computing (SciDAC) Program and by the Office of Science Earth System Modeling Program. Computing resources were provided by the Climate Simulation Laboratory at NCAR's Computational and Information Systems Laboratory (CISL), sponsored by the National Science Foundation and other agencies. The Pacific Northwest National Laboratory is operated for DOE by Battelle Memorial Institute under contract DE-AC06-76RLO 1830. Simulations of the ECHAM5-HAM, INCA, CAM4-Oslo and HadGEM2 models have been supported with funds from the FP6 project EUCAARI (Contract 34684). A. Kirkevag, T. Iversen and O. Seland (CAM4-Oslo) were supported by the Research Council of Norway through the EarthClim (207711/E10) and NOTUR/NorStore projects, by the Norwegian Space Centre through PM-VRAE, and through the EU projects PEGASOS and ACCESS. G. Myhre and B. Samset were funded by the Research Council of Norway through the EarthClim and SLAC projects. K. Tsigaridis and S. Bauer were supported by NASA-MAP (NASA award NNX09AK32G). Resources supporting this work were provided by the NASA High-End Computing (HEC) Program through the NASA Center for Climate Simulation (NCCS) at Goddard Space Flight Center. N. Bellouin was supported by the Joint DECC/Defra Met Office Hadley Centre Climate Programme (GA01101). We also thank the two anonymous reviewers for their efforts. NR 37 TC 63 Z9 67 U1 3 U2 56 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1680-7316 EI 1680-7324 J9 ATMOS CHEM PHYS JI Atmos. Chem. Phys. PY 2013 VL 13 IS 5 BP 2423 EP 2434 DI 10.5194/acp-13-2423-2013 PG 12 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 117NP UT WOS:000316960500008 ER PT J AU Voulgarakis, A Naik, V Lamarque, JF Shindell, DT Young, PJ Prather, MJ Wild, O Field, RD Bergmann, D Cameron-Smith, P Cionni, I Collins, WJ Dalsoren, SB Doherty, RM Eyring, V Faluvegi, G Folberth, GA Horowitz, LW Josse, B MacKenzie, IA Nagashima, T Plummer, DA Righi, M Rumbold, ST Stevenson, DS Strode, SA Sudo, K Szopa, S Zeng, G AF Voulgarakis, A. Naik, V. Lamarque, J. -F. Shindell, D. T. Young, P. J. Prather, M. J. Wild, O. Field, R. D. Bergmann, D. Cameron-Smith, P. Cionni, I. Collins, W. J. Dalsoren, S. B. Doherty, R. M. Eyring, V. Faluvegi, G. Folberth, G. A. Horowitz, L. W. Josse, B. MacKenzie, I. A. Nagashima, T. Plummer, D. A. Righi, M. Rumbold, S. T. Stevenson, D. S. Strode, S. A. Sudo, K. Szopa, S. Zeng, G. TI Analysis of present day and future OH and methane lifetime in the ACCMIP simulations SO ATMOSPHERIC CHEMISTRY AND PHYSICS LA English DT Article ID GENERAL-CIRCULATION MODEL; GLOBAL LIGHTNING DISTRIBUTIONS; CHEMICAL-TRANSPORT MODEL; TROPOSPHERIC OZONE; ATMOSPHERIC CHEMISTRY; HYDROXYL RADICALS; CLIMATE-CHANGE; INTERANNUAL VARIABILITY; STRATOSPHERIC OZONE; PREINDUSTRIAL TIMES AB Results from simulations performed for the Atmospheric Chemistry and Climate Modeling Intercomparison Project (ACCMIP) are analysed to examine how OH and methane lifetime may change from present day to the future, under different climate and emissions scenarios. Present day (2000) mean tropospheric chemical lifetime derived from the ACCMIP multi-model mean is 9.8 +/- 1.6 yr (9.3 +/- 0.9 yr when only including selected models), lower than a recent observationally-based estimate, but with a similar range to previous multi-model estimates. Future model projections are based on the four Representative Concentration Pathways (RCPs), and the results also exhibit a large range. Decreases in global methane lifetime of 4.5 +/- 9.1% are simulated for the scenario with lowest radiative forcing by 2100 (RCP 2.6), while increases of 8.5 +/- 10.4% are simulated for the scenario with highest radiative forcing (RCP 8.5). In this scenario, the key driver of the evolution of OH and methane lifetime is methane itself, since its concentration more than doubles by 2100 and it consumes much of the OH that exists in the troposphere. Stratospheric ozone recovery, which drives tropospheric OH decreases through photolysis modifications, also plays a partial role. In the other scenarios, where methane changes are less drastic, the interplay between various competing drivers leads to smaller and more diverse OH and methane lifetime responses, which are difficult to attribute. For all scenarios, regional OH changes are even more variable, with the most robust feature being the large decreases over the remote oceans in RCP8.5. Through a regression analysis, we suggest that differences in emissions of non-methane volatile organic compounds and in the simulation of photolysis rates may be the main factors causing the differences in simulated present day OH and methane lifetime. Diversity in predicted changes between present day and future OH was found to be associated more strongly with differences in modelled temperature and stratospheric ozone changes. Finally, through perturbation experiments we calculated an OH feedback factor (F) of 1.24 from present day conditions (1.50 from 2100 RCP8.5 conditions) and a climate feedback on methane lifetime of 0.33 +/- 0.13 yr K-1, on average. Models that did not include interactive stratospheric ozone effects on photolysis showed a stronger sensitivity to climate, as they did not account for negative effects of climate-driven stratospheric ozone recovery on tropospheric OH, which would have partly offset the overall OH/methane lifetime response to climate change. C1 [Voulgarakis, A.; Shindell, D. T.; Field, R. D.; Faluvegi, G.] NASA, Goddard Inst Space Studies, New York, NY 10025 USA. [Voulgarakis, A.; Shindell, D. T.; Field, R. D.; Faluvegi, G.] Columbia Earth Inst, New York, NY USA. [Voulgarakis, A.; Eyring, V.] Univ London Imperial Coll Sci Technol & Med, Dept Phys, London, England. [Naik, V.] NOAA, UCAR, Geophys Fluid Dynam Lab, Princeton, NJ USA. [Lamarque, J. -F.] Natl Ctr Atmospher Res, Boulder, CO 80307 USA. [Young, P. J.] Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA. [Young, P. J.] NOAA, Earth Syst Res Lab, Boulder, CO USA. [Young, P. J.; Wild, O.] Univ Lancaster, Lancaster Environm Ctr, Lancaster, England. [Prather, M. J.] Univ Calif Irvine, Irvine, CA USA. [Field, R. D.] Columbia Univ, Dept Appl Phys & Appl Math, New York, NY 10027 USA. [Bergmann, D.; Cameron-Smith, P.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Cionni, I.] Agenzia Nazl Nuove Tecnol, Energia & Sviluppo Econ Sostenibile ENEA, Bologna, Italy. [Collins, W. J.; Folberth, G. A.; Rumbold, S. T.] Met Off Hadley Ctr, Exeter, Devon, England. [Collins, W. J.] Univ Reading, Dept Meteorol, Reading RG6 2AH, Berks, England. [Dalsoren, S. B.] CICERO, Oslo, Norway. [Doherty, R. M.; MacKenzie, I. A.; Stevenson, D. S.] Univ Edinburgh, Edinburgh, Midlothian, Scotland. [Horowitz, L. W.] NOAA, Geophys Fluid Dynam Lab, Princeton, NJ USA. [Josse, B.] CNRS, Meteo France, GAME, Toulouse, France. [Nagashima, T.; Sudo, K.] Natl Inst Environm Studies, Tsukuba, Ibaraki, Japan. [Plummer, D. A.] Environm Canada, Victoria, BC, Canada. [Strode, S. A.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Strode, S. A.] Univ Space Res Assoc, Greenbelt, MD USA. [Szopa, S.] IPSL, UVSQ, CNRS, CEA,LSCE, Paris, France. [Zeng, G.] Natl Inst Water & Atmospher Res, Lauder, New Zealand. RP Voulgarakis, A (reprint author), NASA, Goddard Inst Space Studies, New York, NY 10025 USA. EM a.voulgarakis@imperial.ac.uk RI Strode, Sarah/H-2248-2012; Eyring, Veronika/O-9999-2016; Manager, CSD Publications/B-2789-2015; Righi, Mattia/I-5120-2013; Cameron-Smith, Philip/E-2468-2011; Szopa, Sophie/F-8984-2010; Shindell, Drew/D-4636-2012; Horowitz, Larry/D-8048-2014; Naik, Vaishali/A-4938-2013; Lamarque, Jean-Francois/L-2313-2014; Collins, William/A-5895-2010; Stevenson, David/C-8089-2012; Wild, Oliver/A-4909-2009; mackenzie, ian/E-9320-2013; Bergmann, Daniel/F-9801-2011; Young, Paul/E-8739-2010 OI Strode, Sarah/0000-0002-8103-1663; Eyring, Veronika/0000-0002-6887-4885; Folberth, Gerd/0000-0002-1075-440X; Righi, Mattia/0000-0003-3827-5950; Cameron-Smith, Philip/0000-0002-8802-8627; Szopa, Sophie/0000-0002-8641-1737; Horowitz, Larry/0000-0002-5886-3314; Naik, Vaishali/0000-0002-2254-1700; Lamarque, Jean-Francois/0000-0002-4225-5074; Collins, William/0000-0002-7419-0850; Stevenson, David/0000-0002-4745-5673; Wild, Oliver/0000-0002-6227-7035; Bergmann, Daniel/0000-0003-4357-6301; Young, Paul/0000-0002-5608-8887 FU International Global Atmospheric Chemistry (IGAC) and Stratospheric Processes And their Role in Climate (SPARC) projects under the International Geosphere-Biosphere Project (IGBP); World Climate Research Program (WCRP); U.S. Dept. of Energy (BER); LLNL [DE-AC52-07NA2734]; NERSC [DE11AC02-05CH11231]; Norwegian Research Council; DLR Earth System Model Validation (ESMVal) project; ENEA National Integrated Model to support the international negotiation on atmospheric pollution (Minni) project; NASA Modeling, Analysis and Prediction program; NASA; Joint DECC and Defra Integrated Climate Programme [GA01101]; Meteo-France; CNRS; Environment Research and Technology Development Fund of the Ministry of the Environment, Japan [S-7]; National Science Foundation; Office of 1 Science (BER) of the US Department of Energy; UK research council [NE/I008063/1]; New Zealand Ministry of Science and Innovation FX ACCMIP is organised under the auspices of the International Global Atmospheric Chemistry (IGAC) and Stratospheric Processes And their Role in Climate (SPARC) projects under the International Geosphere-Biosphere Project (IGBP) and World Climate Research Program (WCRP). The authors are grateful to the British Atmospheric Data Centre (BADC), which is part of the NERC National Centre for Atmospheric Science (NCAS), for collecting and archiving the ACCMIP data. For CESM-CAM-superfast, DB and PC were funded by the U.S. Dept. of Energy (BER), performed under the auspices of LLNL under Contract DE-AC52-07NA27344, and used the supercomputing resources of NERSC under contract No. DE11AC02-05CH11231. The CICERO-OsloCTM2 simulations were done within the projects SLAC (Short Lived Atmospheric Components) and EarthClim funded by the Norwegian Research Council. DP would like to thank the Canadian Foundation for Climate and Atmospheric Sciences for their long-running support of CMAM development. For EMAC, the work of VE and MR was funded by the DLR Earth System Model Validation (ESMVal) project and used the supercomputing resources of the German Climate Computing Center (DKRZ) and the Leibniz Supercomputing Centre (LRZ), and the work of IC was funded by the ENEA National Integrated Model to support the international negotiation on atmospheric pollution (Minni) project. The GEOSCCM work was supported by the NASA Modeling, Analysis and Prediction program, with computing resources provided by NASA's High-End Computing Program through the NASA Advanced Supercomputing Division. VN and LWH acknowledge efforts of GFDL's Global Atmospheric Model Development Team in the development of the GFDL-AM3 and Modeling Services Group for assistance with data processing. For the GISS models, support is acknowledged from the NASA MAP and ACMAP programs. For HadGEM2, WJC, GAF, and STR were supported by the Joint DECC and Defra Integrated Climate Programme (GA01101). The LMDz-OR-INCA simulations were done using computing resources provided by the CCRT/GENCI computer center of the CEA. The MOCAGE simulations were supported by Meteo-France and CNRS. Supercomputing time was provided by Meteo-France/DSI supercomputing centre. The MIROC-CHEM calculations were performed on the NIES supercomputer system (NEC SX-8R), and supported by the Environment Research and Technology Development Fund (S-7) of the Ministry of the Environment, Japan. The CESM project, including NCAR-CAM3.5, is supported by the National Science Foundation and the Office of 1 Science (BER) of the US Department of Energy. The National Center for Atmospheric Research is operated by the University Corporation for Atmospheric Research under sponsorship of the National Science Foundation. The STOC-HadAM3 work was supported by cross UK research council grant NE/I008063/1 and used facilities provided by the UK's national high-performance computing service, HECToR, through Computational Modelling Services (CMS), part of the NERC National Centre for Atmospheric Science (NCAS). For UM-CAM, GZ acknowledges NIWA HPCF facility and funding from New Zealand Ministry of Science and Innovation. AV thanks Chris Holmes for clarifications on the observational methane lifetime estimate. NR 97 TC 73 Z9 75 U1 5 U2 61 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1680-7316 EI 1680-7324 J9 ATMOS CHEM PHYS JI Atmos. Chem. Phys. PY 2013 VL 13 IS 5 BP 2563 EP 2587 DI 10.5194/acp-13-2563-2013 PG 25 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 117NP UT WOS:000316960500017 ER PT J AU Lee, YH Lamarque, JF Flanner, MG Jiao, C Shindell, DT Berntsen, T Bisiaux, MM Cao, J Collins, WJ Curran, M Edwards, R Faluvegi, G Ghan, S Horowitz, LW McConnell, JR Ming, J Myhre, G Nagashima, T Naik, V Rumbold, ST Skeie, RB Sudo, K Takemura, T Thevenon, F Xu, B Yoon, JH AF Lee, Y. H. Lamarque, J. -F. Flanner, M. G. Jiao, C. Shindell, D. T. Berntsen, T. Bisiaux, M. M. Cao, J. Collins, W. J. Curran, M. Edwards, R. Faluvegi, G. Ghan, S. Horowitz, L. W. McConnell, J. R. Ming, J. Myhre, G. Nagashima, T. Naik, V. Rumbold, S. T. Skeie, R. B. Sudo, K. Takemura, T. Thevenon, F. Xu, B. Yoon, J. -H. TI Evaluation of preindustrial to present-day black carbon and its albedo forcing from Atmospheric Chemistry and Climate Model Intercomparison Project (ACCMIP) SO ATMOSPHERIC CHEMISTRY AND PHYSICS LA English DT Article ID BIOMASS BURNING EMISSIONS; AEROSOL LIGHT-ABSORPTION; LONG-TERM TRENDS; ICE CORE; ARCTIC SNOW; SOOT; DEPOSITION; TRANSPORT; SIMULATION; PARTICLES AB As part of the Atmospheric Chemistry and Climate Model Intercomparison Project (ACCMIP), we evaluate the historical black carbon (BC) aerosols simulated by 8 ACCMIP models against observations including 12 ice core records, long-term surface mass concentrations, and recent Arctic BC snowpack measurements. We also estimate BC albedo forcing by performing additional simulations using offline models with prescribed meteorology from 1996-2000. We evaluate the vertical profile of BC snow concentrations from these offline simulations using the recent BC snowpack measurements. Despite using the same BC emissions, the global BC burden differs by approximately a factor of 3 among models due to differences in aerosol removal parameterizations and simulated meteorology: 34 Gg to 103 Gg in 1850 and 82 Gg to 315 Gg in 2000. However, the global BC burden from preindustrial to present-day increases by 2.5-3 times with little variation among models, roughly matching the 2.5-fold increase in total BC emissions during the same period. We find a large divergence among models at both Northern Hemisphere (NH) and Southern Hemisphere (SH) high latitude regions for BC burden and at SH high latitude regions for deposition fluxes. The ACCMIP simulations match the observed BC surface mass concentrations well in Europe and North America except at Ispra. However, the models fail to predict the Arctic BC seasonality due to severe under-estimations during winter and spring. The simulated vertically resolved BC snow concentrations are, on average, within a factor of 2-3 of the BC snowpack measurements except for Greenland and the Arctic Ocean. For the ice core evaluation, models tend to adequately capture both the observed temporal trends and the magnitudes at Greenland sites. However, models fail to predict the decreasing trend of BC depositions/ice core concentrations from the 1950s to the 1970s in most Tibetan Plateau ice cores. The distinct temporal trend at the Tibetan Plateau ice cores indicates a strong influence from Western Europe, but the modeled BC increases in that period are consistent with the emission changes in Eastern Europe, the Middle East, South and East Asia. At the Alps site, the simulated BC suggests a strong influence from Europe, which agrees with the Alps ice core observations. At Zuoqiupu on the Tibetan Plateau, models successfully simulate the higher BC concentrations observed during the non-monsoon season compared to the monsoon season but overpredict BC in both seasons. Despite a large divergence in BC deposition at two Antarctic ice core sites, some models with a BC lifetime of less than 7 days are able to capture the observed concentrations. In 2000 relative to 1850, globally and annually averaged BC surface albedo forcing from the offline simulations ranges from 0.014 to 0.019 W m(-2) among the ACCMIP models. Comparing offline and online BC albedo forcings computed by some of the same models, we find that the global annual mean can vary by up to a factor of two because of different aerosol models or different BC-snow parameterizations and snow cover. The spatial distributions of the offline BC albedo forcing in 2000 show especially high BC forcing (i.e., over 0.1 W m(-2)) over Manchuria, Karakoram, and most of the Former USSR. Models predict the highest global annual mean BC forcing in 1980 rather than 2000, mostly driven by the high fossil fuel and biofuel emissions in the Former USSR in 1980. C1 [Lee, Y. H.; Shindell, D. T.; Faluvegi, G.] NASA, Goddard Inst Space Studies, New York, NY 10025 USA. [Lee, Y. H.; Shindell, D. T.; Faluvegi, G.] Columbia Earth Inst, New York, NY USA. [Lamarque, J. -F.] Natl Ctr Atmospher Res, Boulder, CO 80307 USA. [Flanner, M. G.; Jiao, C.] Univ Michigan, Dept Atmospher Ocean & Space Sci, Ann Arbor, MI 48109 USA. [Berntsen, T.; Myhre, G.] CICERO, Oslo, Norway. [Berntsen, T.] Univ Oslo, Dept Geosci, Oslo, Norway. [Bisiaux, M. M.; McConnell, J. R.] Univ Nevada, Desert Res Inst, Nevada Syst Higher Educ, Reno, NV 89506 USA. [Cao, J.] Chinese Acad Sci, Inst Earth Environm, State Key Lab Loess & Quaternary Geol, Xian, Peoples R China. [Collins, W. J.; Rumbold, S. T.] Met Off, Hadley Ctr, Exeter, Devon, England. [Edwards, R.] Curtin Univ Technol, Dept Imaging & Appl Phys, Bentley, WA 6102, Australia. [Ghan, S.; Yoon, J. -H.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Horowitz, L. W.] NOAA, Geophys Fluid Dynam Lab, Princeton, NJ USA. [Ming, J.] China Meteorol Adm, Natl Climate Ctr, Beijing, Peoples R China. [Nagashima, T.; Skeie, R. B.] Natl Inst Environm Studies, Tsukuba, Ibaraki, Japan. [Naik, V.] NOAA, UCAR, Geophys Fluid Dynam Lab, Princeton, NJ USA. [Sudo, K.] Nagoya Univ, Grad Sch Environm Studies, Dept Earth & Environm Sci, Nagoya, Aichi 4648601, Japan. [Takemura, T.] Kyushu Univ, Res Inst Appl Mech, Fukuoka 812, Japan. [Thevenon, F.] Univ Geneva, FA Forel Inst, Versoix, Switzerland. [Xu, B.] Chinese Acad Sci, Inst Tibetan Plateau Res, Key Lab Tibetan Environm Changes & Land Surface P, Beijing, Peoples R China. RP Lee, YH (reprint author), NASA, Goddard Inst Space Studies, New York, NY 10025 USA. EM yunha.lee@nasa.gov RI Collins, William/A-5895-2010; Myhre, Gunnar/A-3598-2008; Skeie, Ragnhild/K-1173-2015; Takemura, Toshihiko/C-2822-2009; Thevenon, Florian/E-3496-2010; Flanner, Mark/C-6139-2011; Shindell, Drew/D-4636-2012; Horowitz, Larry/D-8048-2014; Naik, Vaishali/A-4938-2013; YOON, JIN-HO/A-1672-2009; Lamarque, Jean-Francois/L-2313-2014; Kyushu, RIAM/F-4018-2015; Jiao, Chaoyi/F-9065-2015; U-ID, Kyushu/C-5291-2016; Ghan, Steven/H-4301-2011; Edwards, Ross/B-1433-2013; Lee, Yunha/Q-7222-2016; Cao, Junji/D-3259-2014; OI Collins, William/0000-0002-7419-0850; Myhre, Gunnar/0000-0002-4309-476X; Skeie, Ragnhild/0000-0003-1246-4446; Takemura, Toshihiko/0000-0002-2859-6067; Flanner, Mark/0000-0003-4012-174X; Horowitz, Larry/0000-0002-5886-3314; Naik, Vaishali/0000-0002-2254-1700; YOON, JIN-HO/0000-0002-4939-8078; Lamarque, Jean-Francois/0000-0002-4225-5074; Ghan, Steven/0000-0001-8355-8699; Edwards, Ross/0000-0002-9233-8775; Lee, Yunha/0000-0001-7478-2672; Cao, Junji/0000-0003-1000-7241; Ming, Jing/0000-0001-5527-3768 FU Atmospheric Chemistry and Climate (AC& C), a project of International Global Atmospheric Chemistry (IGAC) and Stratospheric Processes And their Role in Climate (SPARC); NASA; US Department of Energy Office of Science Decadal and Regional Climate Prediction using Earth System Models (EaSM) program; Department of Energy (DOE) by Battelle Memorial Institute [DE-AC06-76RLO 1830]; Joint DECC and Defra Integrated Climate Programme [GA01101]; Norwegian Research Council; National Science Foundation; Office of Science (BER) of the US Department of Energy; Environment Research and Technology Development Fund of the Ministry of the Environment, Japan [S7]; NILU; Norsk Polar Institute FX ACCMIP is organized under the auspices of Atmospheric Chemistry and Climate (AC& C), a project of International Global Atmospheric Chemistry (IGAC) and Stratospheric Processes And their Role in Climate (SPARC) under the International Geosphere-Biosphere Project (IGBP) andWorld Climate Research Program (WCRP). The authors are thankful to the British Atmospheric Data Centre (BADC), which is part of the NERC National Centre for Atmospheric Science (NCAS), for collecting and archiving the ACCMIP data. Y. H. Lee, D. T. Shindell, and G. Faluvegi acknowledge the support of the NASA MAP and ACMAP programs. Resources supporting the two GISS models simulations were provided by the NASA High-End Computing (HEC) Program through the NASA Center for Climate Simulation (NCCS) at Goddard Space Flight Center. V. Naik and L. W. Horowitz acknowledge the efforts of GFDL's Global Atmospheric Model Development Team in the development of the GFDL-AM3 and the efforts of the Modeling Services Group for assistance with data processing. S. Ghan and J.-H. Yoon were supported by the US Department of Energy Office of Science Decadal and Regional Climate Prediction using Earth System Models (EaSM) program. The Pacific Northwest National Laboratory (PNNL) is operated for the Department of Energy (DOE) by Battelle Memorial Institute under contract DE-AC06-76RLO 1830. W. J. Collins and S. T. Rumbold were supported by the Joint DECC and Defra Integrated Climate Programme (GA01101). The CICERO-OsloCTM2 simulations were done within the projects SLAC (Short Lived Atmospheric Components) and EarthClim funded by the Norwegian Research Council. The CESM project, including NCAR-CAM3.5, is supported by the National Science Foundation and the Office of Science (BER) of the US Department of Energy. The National Center for Atmospheric Research is operated by the University Corporation for Atmospheric Research under sponsorship of the National Science Foundation. The MIROC-CHEM calculations were performed on the NIES supercomputer system (NEC SX-8R) and supported by the Environment Research and Technology Development Fund (S7) of the Ministry of the Environment, Japan. Development of historical records of BC in Greenland and Antarctic ice cores was funded by the National Science Foundation.; The authors would like to thank NOAA-ESRL-GMD aerosol group, Norwegian Institute for Air Research (NILU), Atmospheric Radiation Measurement (ARM) Climate Research Facility operated for DOE, Sangeeta Sharma (Environment Canada), Heikki Lihavainen (Finnish Meteorological Institute), Sandy Starkweather (NOAA), Ernest Weingartner (Paul Scherrer Institute), and Martine Collaud Coen (MeteoSwiss) for providing BC surface mass concentration data. Special thanks to Betsy Andrews at NOAA and Ann Mari Fj raa at NILU for helping us to obtain several BC surface mass concentrations datasets. We thank the EUSAAR-ACTRIS network for sampling BC at several EMEP stations. S. G. Jennings and Colin O'Dowd, Centre for Climate and Air Pollution Studies, School of Physics, National University of Ireland Galway are acknowledged for the use of surface black carbon data taken at the Mace Head Atmospheric Research Station on the west coast of Ireland. We also acknowledge the contribution of aethalometer BC data from Zeppelin, Ny-A lesund by K. Eleftheriadis, NCSR Demokritos and the support of NILU and Norsk Polar Institute. Finally, special thanks to Stephen Warren (Dept. of Atmospheric Science, Univ. ofWashington, Seattle, WA, USA) and Sarah Doherty (JISAO, Univ. of Washington, Seattle, WA, USA) for making available measurements of snow BC concentrations from the Arctic. NR 102 TC 47 Z9 53 U1 10 U2 73 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1680-7316 EI 1680-7324 J9 ATMOS CHEM PHYS JI Atmos. Chem. Phys. PY 2013 VL 13 IS 5 BP 2607 EP 2634 DI 10.5194/acp-13-2607-2013 PG 28 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 117NP UT WOS:000316960500019 ER PT J AU Vent-Schmidt, T Hunt, RD Andrews, L Riedel, S AF Vent-Schmidt, Thomas Hunt, Rodney Dale Andrews, Lester Riedel, Sebastian TI Formation and characterization of HUF and DUF in solid argon SO CHEMICAL COMMUNICATIONS LA English DT Article ID TRANSFORM INFRARED-SPECTRA; BOND COVALENT RADII; URANIUM; MOLECULES; THERMOCHEMISTRY; COMPLEXES AB Reactions of laser-ablated U atoms with HF and DF in condensing and solid rare gas produce HUF and DUF as the major new products based on close agreement between observed and calculated vibrational frequencies and deuterium shifts for U-H and U-F stretching modes at 1383 and 544 cm(-1), respectively. C1 [Vent-Schmidt, Thomas; Andrews, Lester; Riedel, Sebastian] Univ Freiburg, Inst Anorgan & Analyt Chem, D-79104 Freiburg, Germany. [Hunt, Rodney Dale] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Andrews, Lester] Univ Virginia, Dept Chem, Charlottesville, VA 22904 USA. RP Andrews, L (reprint author), Univ Freiburg, Inst Anorgan & Analyt Chem, Albertstr 21, D-79104 Freiburg, Germany. EM huntrd@ornl.gov; lsa@virginia.edu; sriedel@psichem.de FU DOE [DE-SC0001034]; Fonds der Chemischen Industrie (FCI) FX We gratefully acknowledge financial support from DOE Grant No. DE-SC0001034 to LA. SR thanks the Fonds der Chemischen Industrie (FCI) for financial support. We are grateful to Prof. Ingo Krossing and Prof. Harald Hillebrecht for their generous and continuous support. The authors are also grateful to Dr. Florian Kraus for the donation of uranium metal. NR 22 TC 6 Z9 6 U1 2 U2 9 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1359-7345 J9 CHEM COMMUN JI Chem. Commun. PY 2013 VL 49 IS 37 BP 3863 EP 3865 DI 10.1039/c3cc41379a PG 3 WC Chemistry, Multidisciplinary SC Chemistry GA 122YA UT WOS:000317353300012 PM 23538396 ER PT J AU Sun, YG AF Sun, Yugang TI Controlled synthesis of colloidal silver nanoparticles in organic solutions: empirical rules for nucleation engineering SO CHEMICAL SOCIETY REVIEWS LA English DT Review ID ENHANCED RAMAN-SPECTROSCOPY; METAL NANOPARTICLES; OXIDATION REACTIONS; ASSISTED SYNTHESIS; MEDIATED SYNTHESIS; POLYOL SYNTHESIS; SIZE-DEPENDENCE; SINGLE-CRYSTAL; NANOSTRUCTURES; SHAPE AB Controlled synthesis of colloidal nanoparticles in organic solutions is among the most intensely studied topics in nanoscience because of the intrinsic advantages in terms of high yield and high uniformity in comparison with aqueous synthesis. However, systematic studies on the formation mechanism of nanoparticles with precisely tailored physical parameters are barely reported. In this tutorial review, we take the synthesis of different Ag nanoparticles as an example to rule out the general principles for controlling the nucleation process involved in the formation of colloidal Ag nanoparticles in organic solutions, which enables the synthesis of high-quality nanoparticles. C1 Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. RP Sun, YG (reprint author), Argonne Natl Lab, Ctr Nanoscale Mat, 9700 S Cass Ave, Argonne, IL 60439 USA. EM ygsun@anl.gov RI Sun, Yugang /A-3683-2010 OI Sun, Yugang /0000-0001-6351-6977 FU Center for Nanoscale Materials, a U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility [DE-AC02-06CH11357]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work was performed at the Center for Nanoscale Materials, a U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility under Contract No. DE-AC02-06CH11357. Data discussed in this review were partially obtained with the use of Advanced Photon Source and Electron Microscopy Center for Materials Research at Argonne National Laboratory that are supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. Dr Sheng Peng's efforts on the synthesis of Ag icosahedral nanoparticles, Ag nanocubes, and Ag/FexOy hybrid nanoparticles are greatly appreciated. NR 75 TC 73 Z9 74 U1 7 U2 190 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 0306-0012 J9 CHEM SOC REV JI Chem. Soc. Rev. PY 2013 VL 42 IS 7 BP 2497 EP 2511 DI 10.1039/c2cs35289c PG 15 WC Chemistry, Multidisciplinary SC Chemistry GA 116FX UT WOS:000316869500003 PM 23072940 ER PT J AU Wang, C Takei, K Takahashi, T Javey, A AF Wang, Chuan Takei, Kuniharu Takahashi, Toshitake Javey, Ali TI Carbon nanotube electronics - moving forward SO CHEMICAL SOCIETY REVIEWS LA English DT Review ID THIN-FILM TRANSISTORS; FIELD-EFFECT TRANSISTORS; CHEMICAL-VAPOR-DEPOSITION; LIGHT-EMITTING DEVICES; ALIGNED ARRAYS; INTEGRATED-CIRCUITS; RADIOFREQUENCY APPLICATIONS; ORGANIC TRANSISTORS; RADIO-FREQUENCY; RANDOM NETWORKS AB Single-walled carbon nanotubes (SWNTs) possess fascinating electrical properties and offer new entries into a wide range of novel electronic applications that are unattainable with conventional Si-based devices. The field initially focused on the use of individual or parallel arrays of nanotubes as the channel material for ultra-scaled nanoelectronic devices. However, the challenge in the deterministic assembly has proven to be a major technological barrier. In recent years, solution deposition of semiconductor-enriched SWNT networks has been actively explored for high performance and uniform thin-film transistors (TFTs) on mechanically rigid and flexible substrates. This presents a unique niche for nanotube electronics by overcoming their limitations and taking full advantage of their superb chemical and physical properties. This review focuses on the large-area processing and electronic properties of SWNT TFTs. A wide range of applications in conformal integrated circuits, radio-frequency electronics, artificial skin sensors, and displays are discussed - with emphasis on large-area systems where nm-scale accuracy in the assembly of nanotubes is not required. The demonstrations show SWNTs' immense promise as a low-cost and scalable TFT technology for nonconventional electronic systems with excellent device performances. C1 [Wang, Chuan; Takei, Kuniharu; Takahashi, Toshitake; Javey, Ali] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Wang, Chuan; Takei, Kuniharu; Takahashi, Toshitake; Javey, Ali] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Javey, A (reprint author), Univ Calif Berkeley, Berkeley, CA 94720 USA. EM ajavey@eecs.berkeley.edu RI Wang, Chuan/B-3649-2011; Javey, Ali/B-4818-2013 FU NSF COINS; NSF CAREER Award; DARPA/DSO Maximum Mobility and Manipulation; World Class University program at Sunchon National University; Sloan Fellowship FX This work was partially funded by NSF COINS, NSF CAREER Award, and DARPA/DSO Maximum Mobility and Manipulation. A.J. acknowledges support from the World Class University program at Sunchon National University and a Sloan Fellowship. NR 94 TC 126 Z9 126 U1 17 U2 253 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 0306-0012 J9 CHEM SOC REV JI Chem. Soc. Rev. PY 2013 VL 42 IS 7 BP 2592 EP 2609 DI 10.1039/c2cs35325c PG 18 WC Chemistry, Multidisciplinary SC Chemistry GA 116FX UT WOS:000316869500009 PM 23229523 ER PT J AU Kao, J Thorkelsson, K Bai, P Rancatore, BJ Xu, T AF Kao, Joseph Thorkelsson, Kari Bai, Peter Rancatore, Benjamin J. Xu, Ting TI Toward functional nanocomposites: taking the best of nanoparticles, polymers, and small molecules SO CHEMICAL SOCIETY REVIEWS LA English DT Review ID COPOLYMER THIN-FILMS; LIQUID-CRYSTALLINE POLYMERS; COMB-SHAPED SUPRAMOLECULES; SELF-ASSEMBLED STRUCTURES; COIL DIBLOCK COPOLYMERS; SEPARATED BLOCK-COPOLYMERS; MAGNETIC-FIELD ALIGNMENT; 2 LENGTH SCALES; GOLD NANORODS; SIDE-CHAIN AB Nanocomposites, composed of organic and inorganic building blocks, can combine the properties from the parent constituents and generate new properties to meet current and future demands in functional materials. Recent developments in nanoparticle synthesis provide a plethora of inorganic building blocks, building the foundation for constructing hybrid nanocomposites with unlimited possibilities. The properties of nanocomposite materials depend not only on those of individual building blocks but also on their spatial organization at different length scales. Block copolymers, which microphase separate into various nanostructures, have shown their potential for organizing inorganic nanoparticles in bulk/thin films. Block copolymer-based supramolecules further provide more versatile routes to control spatial arrangement of the nanoparticles over multiple length scales. This review provides an overview of recent efforts to control the hierarchical assemblies in block copolymer-based hybrid nanocomposites. C1 [Kao, Joseph; Thorkelsson, Kari; Bai, Peter; Xu, Ting] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Rancatore, Benjamin J.; Xu, Ting] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Xu, Ting] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA USA. RP Xu, T (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. EM tingxu@berkeley.edu RI Bai, Peter/J-9084-2014 NR 271 TC 145 Z9 146 U1 22 U2 440 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 0306-0012 EI 1460-4744 J9 CHEM SOC REV JI Chem. Soc. Rev. PY 2013 VL 42 IS 7 BP 2654 EP 2678 DI 10.1039/c2cs35375j PG 25 WC Chemistry, Multidisciplinary SC Chemistry GA 116FX UT WOS:000316869500011 PM 23192158 ER PT J AU Wang, T LaMontagne, D Lynch, J Zhuang, JQ Cao, YC AF Wang, Tie LaMontagne, Derek Lynch, Jared Zhuang, Jiaqi Cao, Y. Charles TI Colloidal superparticles from nanoparticle assembly SO CHEMICAL SOCIETY REVIEWS LA English DT Review ID NANOCRYSTAL SUPERLATTICE MEMBRANES; UNIFORM COLLOIDS; QUANTUM DOTS; SEMICONDUCTOR NANOCRYSTALS; DIFFUSIONAL NUCLEATION; SELECTIVE ENRICHMENT; NANOSIZE PRECURSORS; CLUSTERS; SHAPE; CRYSTALLIZATION AB Colloidal superparticles are size- and shape-controlled nanoparticle assemblies in the form of colloidal particles. Because these superparticles can exhibit physical and chemical properties different from both individual nanoparticles and their bulk assemblies, the development of superparticle synthesis has attracted significant research attention and is emerging as a new frontier in the field of nanotechnology. In this review, we discuss theoretical considerations on the nucleation and growth of colloidal superparticles. We then present recent progress in the synthesis and characterization of monodispersed colloidal superparticles, which are important for applications such as biomedical diagnosis, biological separation, and light emitting devices. C1 [Wang, Tie; LaMontagne, Derek; Cao, Y. Charles] Univ Florida, Dept Chem, Gainesville, FL 32611 USA. [Lynch, Jared] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Zhuang, Jiaqi] Jilin Univ, Changchun 130023, Peoples R China. RP Cao, YC (reprint author), Univ Florida, Dept Chem, Gainesville, FL 32611 USA. EM cao@chem.ufl.edu RI Wang, Tie/L-5060-2015 OI Wang, Tie/0000-0001-5965-6520 FU Office of Naval Research [N00014-09-1-0441]; National Science Foundation [DMR-0645520]; National Nature Science Foundation of China [50902058] FX Y.C.C. acknowledges funding support from the Office of Naval Research (N00014-09-1-0441) and the National Science Foundation (DMR-0645520 Career Award); J. Q. Zhuang acknowledges funding support from the National Nature Science Foundation of China (No.50902058). NR 80 TC 81 Z9 81 U1 28 U2 351 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 0306-0012 J9 CHEM SOC REV JI Chem. Soc. Rev. PY 2013 VL 42 IS 7 BP 2804 EP 2823 DI 10.1039/c2cs35318k PG 20 WC Chemistry, Multidisciplinary SC Chemistry GA 116FX UT WOS:000316869500016 PM 23104182 ER PT J AU Alkalay, A Rabinovici, GD Zimmerman, G Agarwal, N Kaufer, D Miller, BL Jagust, WJ Soreq, H AF Alkalay, Adi Rabinovici, Gil D. Zimmerman, Gabriel Agarwal, Neha Kaufer, Daniela Miller, Bruce L. Jagust, William J. Soreq, Hermona TI Plasma Acetylcholinesterase Activity Correlates with Intracerebral beta-Amyloid Load SO CURRENT ALZHEIMER RESEARCH LA English DT Article DE Amyloid-beta; Pittsburgh Compound-B; amyloid imaging; plasma acetylcholinesterase; plasma butyrylcholinesterase ID CEREBROSPINAL-FLUID-ACETYLCHOLINESTERASE; LONG-TERM TREATMENT; ALZHEIMERS-DISEASE; BUTYRYLCHOLINESTERASE ACTIVITY; IN-VIVO; DEMENTIA; BRAIN; INFLAMMATION; INHIBITORS; RISK AB Background: Previous studies have demonstrated alterations in the peripheral cholinergic system in Alzheimer's disease (AD), though results have been inconsistent and not linked to in vivo biomarkers of pathology. We examined the relationship between amyloid-beta (A beta) plaques and plasma cholinesterase activity in a heterogeneous dementia population. Methods: 29 participants with clinical AD and 35 with non-AD diagnoses underwent positron emission tomography (PET) with the amyloid ligand [11C] PIB and plasma measurements of acetylcholinesterase (AChE) and butyrylcholinesterase (BChE) activity. Multi-linear regression was used to evaluate the relationship between AChE or BChE activity and PIB binding (adjusted for age, sex, apolipoprotein E4 and vascular risk), applying voxel-wise and region of interest (ROI) approaches. AChE activity was further adjusted for cholinesterase inhibitor (ChE-I) use. Global amyloid load was measured using a PIB Index, representing mean tracer binding in frontal, parietal, lateral temporal and cingulate cortex. Results: AChE activity was correlated with PIB Index (beta=0.39, p<0.001) and with regional PIB binding in frontal, temporal, parietal and occipital lobes, precuneus and posterior cingulate on both voxel-wise (p<0.001 uncorrected) and ROI (beta=0.26-0.41, p<0.005) analysis. Correlations remained significant after covarying clinical diagnosis (beta=0.42, p=0.001), and among participants naive to ChE-I (beta=0.51, p=0.005). No correlation was found between BChE activity and PIB. Among AD participants, disease severity was not correlated with AChE, BChE or PIB Index. Conclusion: AChE activity in plasma is correlated with brain A beta load. Activation of the 'anti-inflammatory cholinergic pathway' may provide the link between A beta plaques and peripheral cholinergic measures. C1 [Alkalay, Adi; Rabinovici, Gil D.; Agarwal, Neha; Jagust, William J.] Univ Calif Berkeley, Helen Wills Neurosci Inst, Berkeley, CA 94720 USA. [Alkalay, Adi; Rabinovici, Gil D.; Miller, Bruce L.] Univ Calif San Francisco, Memory & Aging Ctr, San Francisco, CA 94143 USA. [Alkalay, Adi; Rabinovici, Gil D.; Miller, Bruce L.] Univ Calif San Francisco, Dept Neurol, San Francisco, CA 94143 USA. [Alkalay, Adi; Rabinovici, Gil D.; Miller, Bruce L.] Lawrence Berkeley Natl Lab, Berkeley, CA USA. [Zimmerman, Gabriel; Soreq, Hermona] Hebrew Univ Jerusalem, Dept Biol Chem, IL-91904 Jerusalem, Israel. [Zimmerman, Gabriel; Soreq, Hermona] Hebrew Univ Jerusalem, Edmond & Lily Safra Ctr Brain Sci, IL-91904 Jerusalem, Israel. [Kaufer, Daniela] Univ Calif Berkeley, Dept Integrat Biol, Berkeley, CA 94720 USA. RP Soreq, H (reprint author), Hebrew Univ Jerusalem, Dept Biol Chem, IL-91904 Jerusalem, Israel. EM soreq@cc.huji.ac.il FU Rosetrees Foundation; Senior Miller fellowship; ICNC pre-doctoral fellowship; National Institute on Aging [K23-AG031861, R01-AG034570, P01-AG1972403, P50-AG023501]; Alzheimer's Association [NIRG-07-59422, ZEN-08-87090]; John Douglas French Alzheimer's Foundation; State of California Department of Health Services Alzheimer's Disease Research Center of California [04-33516] FX This study was supported by the Rosetrees Foundation and a Senior Miller fellowship (to H.S for work at UCB); an ICNC pre-doctoral fellowship (to G.Z); National Institute on Aging (grant numbers K23-AG031861 to G.D.R, R01-AG034570 to W.J.J, P01-AG1972403 and P50-AG023501 to B.L.M.); Alzheimer's Association (grant numbers NIRG-07-59422 to G.D.R. and ZEN-08-87090 to W.J.J); John Douglas French Alzheimer's Foundation (to G.D.R.) and State of California Department of Health Services Alzheimer's Disease Research Center of California (grant number 04-33516 to B.L.M). NR 52 TC 12 Z9 12 U1 2 U2 8 PU BENTHAM SCIENCE PUBL LTD PI SHARJAH PA EXECUTIVE STE Y-2, PO BOX 7917, SAIF ZONE, 1200 BR SHARJAH, U ARAB EMIRATES SN 1567-2050 J9 CURR ALZHEIMER RES JI Curr. Alzheimer Res. PD JAN PY 2013 VL 10 IS 1 BP 48 EP 56 PG 9 WC Clinical Neurology; Neurosciences SC Neurosciences & Neurology GA 121VE UT WOS:000317271800007 PM 23157337 ER PT J AU Chen, Z Fang, HE Shen, LM Zhang, HW Zhuang, Z AF Chen, Z. Fang, H. E. Shen, L. M. Zhang, H. W. Zhuang, Z. TI SPECIAL ISSUE BASED ON THE MINI-SYMPOSIUM ENTITLED "BIO- AND NANO-MECHANICS AND MATERIALS WITH APPLICATIONS" FOR THE 9TH WORLD CONGRESS ON COMPUTATIONAL MECHANICS (WCCM 2010) FOREWORD SO INTERNATIONAL JOURNAL FOR MULTISCALE COMPUTATIONAL ENGINEERING LA English DT Editorial Material C1 [Chen, Z.] Univ Missouri, Dept Civil & Environm Engn, Columbia, MO 65211 USA. [Fang, H. E.] Sandia Natl Labs, Computat Mat Sci & Engn Dept, Albuquerque, NM 87185 USA. [Shen, L. M.] Univ Sydney, Sch Civil Engn, Sydney, NSW 2006, Australia. [Zhang, H. W.] Dalian Univ Technol, Dept Engn Mech, Dalian 116024, Peoples R China. [Zhuang, Z.] Tsinghua Univ, Dept Engn Mech, Beijing 100084, Peoples R China. RP Chen, Z (reprint author), Univ Missouri, Dept Civil & Environm Engn, Columbia, MO 65211 USA. EM chenzh@missouri.edu RI Shen, Luming/D-1581-2010 NR 0 TC 0 Z9 0 U1 0 U2 5 PU BEGELL HOUSE INC PI REDDING PA 50 CROSS HIGHWAY, REDDING, CT 06896 USA SN 1543-1649 J9 INT J MULTISCALE COM JI Int. J. Multiscale Comput. Eng. PY 2013 VL 11 IS 1 SI SI BP VII EP VIII PG 2 WC Engineering, Multidisciplinary; Mathematics, Interdisciplinary Applications SC Engineering; Mathematics GA 121NL UT WOS:000317251400001 ER PT J AU Billups, SC Larson, J Graf, P AF Billups, Stephen C. Larson, Jeffrey Graf, Peter TI DERIVATIVE-FREE OPTIMIZATION OF EXPENSIVE FUNCTIONS WITH COMPUTATIONAL ERROR USING WEIGHTED REGRESSION SO SIAM JOURNAL ON OPTIMIZATION LA English DT Article DE derivative-free optimization; weighted regression models; noisy function evaluations ID INTERPOLATION; MINIMIZATION; ALGORITHMS; SOFTWARE; GEOMETRY; SETS AB We propose a derivative-free algorithm for optimizing computationally expensive functions with computational error. The algorithm is based on the trust region regression method by Conn, Scheinberg, and Vicente [A. R. Conn, K. Scheinberg, and L. N. Vicente, IMA J. Numer. Anal., 28 (2008), pp. 721-748] but uses weighted regression to obtain more accurate model functions at each trust region iteration. A heuristic weighting scheme is proposed that simultaneously handles (i) differing levels of uncertainty in function evaluations and (ii) errors induced by poor model fidelity. We also extend the theory of Lambda-poisedness and strong Lambda-poisedness to weighted regression. We report computational results comparing interpolation, regression, and weighted regression methods on a collection of benchmark problems. Weighted regression appears to outperform interpolation and regression models on nondifferentiable functions and functions with deterministic noise. C1 [Billups, Stephen C.] Univ Colorado, Dept Math & Stat Sci, Denver, CO 80217 USA. [Larson, Jeffrey] Royal Inst Technol KTH, Sch Elect Engn, SE-10044 Stockholm, Sweden. [Graf, Peter] Natl Renewable Energy Lab, Computat Sci Ctr, Golden, CO 80401 USA. RP Billups, SC (reprint author), Univ Colorado, Dept Math & Stat Sci, Denver, CO 80217 USA. EM Stephen.Billups@ucdenver.edu; jeffreyl@kth.se; Peter.Graf@nrel.gov RI Billups, Stephen/K-5074-2015 OI Billups, Stephen/0000-0003-3627-0793 FU National Science Foundation grant [GK-12-0742434] FX Received by the editors November 12, 2010; accepted for publication (in revised form) September 19, 2012; published electronically January 10, 2013. This research was partially supported by National Science Foundation grant GK-12-0742434. The U.S. Government retains a nonexclusive, royalty-free license to publish or reproduce the published form of this contribution, or allow others to do so, for U.S. Government purposes. Copyright is owned by SIAM to the extent not limited by these rights.; School of Electrical Engineering, Royal Institute of Technology (KTH), SE-10044 Stockholm, Sweden (jeffreyl@kth.se). This author's research was partially supported by National Science Foundation grant GK-12-0742434. NR 27 TC 6 Z9 6 U1 2 U2 8 PU SIAM PUBLICATIONS PI PHILADELPHIA PA 3600 UNIV CITY SCIENCE CENTER, PHILADELPHIA, PA 19104-2688 USA SN 1052-6234 J9 SIAM J OPTIMIZ JI SIAM J. Optim. PY 2013 VL 23 IS 1 BP 27 EP 53 DI 10.1137/100814688 PG 27 WC Mathematics, Applied SC Mathematics GA 116BN UT WOS:000316857500002 ER PT J AU Walker, BN Antonakos, C Retterer, ST Vertes, A AF Walker, Bennett N. Antonakos, Cory Retterer, Scott T. Vertes, Akos TI Metabolic Differences in Microbial Cell Populations Revealed by Nanophotonic Ionization SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE cellular differences; mass spectrometry; metabolites; nanostructures; single-cell analysis ID MASS-SPECTROMETRY; SACCHAROMYCES-CEREVISIAE; QUANTITATIVE-ANALYSIS; FUNCTIONAL GENOMICS; BIOLOGICAL NOISE; ION PRODUCTION; YEAST; MS; RECONSTRUCTION; PHENOTYPES C1 [Walker, Bennett N.; Antonakos, Cory; Vertes, Akos] George Washington Univ, Dept Chem, Washington, DC 20052 USA. [Retterer, Scott T.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Vertes, A (reprint author), George Washington Univ, Dept Chem, Washington, DC 20052 USA. EM vertes@gwu.edu RI Retterer, Scott/A-5256-2011; Vertes, Akos/B-7159-2008 OI Retterer, Scott/0000-0001-8534-1979; Vertes, Akos/0000-0001-5186-5352 FU Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-FG02-01ER15129]; Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX Support from the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences of the U.S. Department of Energy (Grant DE-FG02-01ER15129) is gratefully acknowledged. A portion of this research (nanofabrication) was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. NR 43 TC 12 Z9 12 U1 5 U2 55 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PY 2013 VL 52 IS 13 BP 3650 EP 3653 DI 10.1002/anie.201207348 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA 112WQ UT WOS:000316625400018 PM 23447072 ER PT J AU Zhang, S Metin, O Su, D Sun, SH AF Zhang, Sen Metin, Onder Su, Dong Sun, Shouheng TI Monodisperse AgPd Alloy Nanoparticles and Their Superior Catalysis for the Dehydrogenation of Formic Acid SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE alloys; heterogeneous catalysis; hydrogen storage; nanoparticles ID HYDROGEN GENERATION; AMBIENT CONDITIONS; OXYGEN REDUCTION; ROOM-TEMPERATURE; PD NANOPARTICLES; STORAGE MATERIAL; FUEL-CELLS; DECOMPOSITION; CORE; FUTURE C1 [Zhang, Sen; Metin, Onder; Sun, Shouheng] Brown Univ, Dept Chem, Providence, RI 02912 USA. [Metin, Onder] Ataturk Univ, Fac Sci, Dept Chem, TR-25240 Erzurum, Turkey. [Su, Dong] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Metin, O (reprint author), Brown Univ, Dept Chem, Providence, RI 02912 USA. EM ometin@atauni.edu.tr; ssun@brown.edu RI Zhang, Sen/E-4226-2015; Su, Dong/A-8233-2013 OI Su, Dong/0000-0002-1921-6683 FU U.S. Army Research Laboratory; U.S. Army Research Office under the Multi University Research Initiative (MURI) [W911NF-11-1-0353]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX This work was supported by the U.S. Army Research Laboratory and the U.S. Army Research Office under the Multi University Research Initiative (MURI, grant number W911NF-11-1-0353) on "Stress-Controlled Catalysis via Engineered Nanostructures". Partial work carried out at the Center for Functional Nanomaterials, Brookhaven National Laboratory, was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under contract number DE-AC02-98CH10886. NR 25 TC 117 Z9 119 U1 27 U2 293 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PY 2013 VL 52 IS 13 BP 3681 EP 3684 DI 10.1002/anie.201300276 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA 112WQ UT WOS:000316625400025 PM 23426846 ER PT S AU Campisi, J AF Campisi, Judith BE Julius, D TI Aging, Cellular Senescence, and Cancer SO ANNUAL REVIEW OF PHYSIOLOGY, VOL 75 SE Annual Review of Physiology LA English DT Review; Book Chapter DE antagonistic pleiotropy; DNA damage; inflammation; stress response; tumor suppression ID DNA-DAMAGE-RESPONSE; ONCOGENE-INDUCED SENESCENCE; INFLAMMATORY CYTOKINE SECRETION; STRESS-INDUCED SENESCENCE; PRIMARY HUMAN FIBROBLASTS; DOUBLE-STRAND BREAKS; IN-VIVO; REPLICATIVE SENESCENCE; PREMATURE SENESCENCE; TUMOR SUPPRESSION AB For most species, aging promotes a host of degenerative pathologies that are characterized by debilitating losses of tissue or cellular function. However, especially among vertebrates, aging also promotes hyperplastic pathologies, the most deadly of which is cancer. In contrast to the loss of function that characterizes degenerating cells and tissues, malignant (cancerous) cells must acquire new (albeit aberrant) functions that allow them to develop into a lethal tumor. This review discusses the idea that, despite seemingly opposite characteristics, the degenerative and hyperplastic pathologies of aging are at least partly linked by a common biological phenomenon: a cellular stress response known as cellular senescence. The senescence response is widely recognized as a potent tumor suppressive mechanism. However, recent evidence strengthens the idea that it also drives both degenerative and hyperplastic pathologies, most likely by promoting chronic inflammation. Thus, the senescence response may be the result of antagonistically pleiotropic gene action. C1 [Campisi, Judith] Buck Inst Res Aging, Novato, CA 94945 USA. [Campisi, Judith] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Campisi, J (reprint author), Buck Inst Res Aging, Novato, CA 94945 USA. EM jcampisi@buckinstitute.org FU NIA NIH HHS [P01 AG017242, P01 AG041122, R37 AG009909] NR 150 TC 350 Z9 363 U1 16 U2 110 PU ANNUAL REVIEWS PI PALO ALTO PA 4139 EL CAMINO WAY, PO BOX 10139, PALO ALTO, CA 94303-0897 USA SN 0066-4278 BN 978-0-8243-0375-4 J9 ANNU REV PHYSIOL JI Annu. Rev. Physiol. PY 2013 VL 75 BP 685 EP 705 DI 10.1146/annurev-physiol-030212-183653 PG 21 WC Physiology SC Physiology GA BEF28 UT WOS:000316381400031 PM 23140366 ER PT J AU Biraud, SC Torn, MS Smith, JR Sweeney, C Riley, WJ Tans, PP AF Biraud, S. C. Torn, M. S. Smith, J. R. Sweeney, C. Riley, W. J. Tans, P. P. TI A multi-year record of airborne CO2 observations in the US Southern Great Plains SO ATMOSPHERIC MEASUREMENT TECHNIQUES LA English DT Article ID ATMOSPHERIC CARBON-DIOXIDE; TRANSPORT MODELS; BOUNDARY-LAYER; FLUXES; EXCHANGE; CYCLE; VARIABILITY; INVERSION; SINKS; DELTA-C-13 AB We report on 10 yr of airborne measurements of atmospheric CO2 mole fraction from continuous and flask systems, collected between 2002 and 2012 over the Atmospheric Radiation Measurement Program Climate Research Facility in the US Southern Great Plains (SGP). These observations were designed to quantify trends and variability in atmospheric mole fraction of CO2 and other greenhouse gases with the precision and accuracy needed to evaluate ground-based and satellite-based column CO2 estimates, test forward and inverse models, and help with the interpretation of ground-based CO2 mole-fraction measurements. During flights, we measured CO2 and meteorological data continuously and collected flasks for a rich suite of additional gases: CO2, CO, CH4, N2O, (CO2)-C-13, carbonyl sulfide (COS), and trace hydrocarbon species. These measurements were collected approximately twice per week by small aircraft (Cessna 172 initially, then Cessna 206) on a series of horizontal legs ranging in altitude from 460 m to 5500 m a.m.s.l. Since the beginning of the program, more than 400 continuous CO2 vertical profiles have been collected (2007-2012), along with about 330 profiles from NOAA/ESRL 12-flask (2006-2012) and 284 from NOAA/ESRL 2-flask (2002-2006) packages for carbon cycle gases and isotopes. Averaged over the entire record, there were no systematic differences between the continuous and flask CO2 observations when they were sampling the same air, i.e., over the one-minute flask-sampling time. Using multiple technologies (a flask sampler and two continuous analyzers), we documented a mean difference of < 0.2 ppm between instruments. However, flask data were not equivalent in all regards; horizontal variability in CO2 mole fraction within the 5-10 min legs sometimes resulted in significant differences between flask and continuous measurement values for those legs, and the information contained in fine-scale variability about atmospheric transport was not captured by flask-based observations. The CO2 mole fraction trend at 3000 m a.m.s.l. was 1.91 ppm yr(-1) between 2008 and 2010, very close to the concurrent trend at Mauna Loa of 1.95 ppm yr(-1). The seasonal amplitude of CO2 mole fraction in the free troposphere (FT) was half that in the planetary boundary layer (PBL) (similar to 15 ppm vs. similar to 30 ppm) and twice that at Mauna Loa (approximately 8 ppm). The CO2 horizontal variability was up to 10 ppm in the PBL and less than 1 ppm at the top of the vertical profiles in the FT. C1 [Biraud, S. C.; Torn, M. S.; Riley, W. J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Smith, J. R.] Atmospher Observing Syst Inc, Boulder, CO USA. [Sweeney, C.; Tans, P. P.] NOAA Earth Syst Res Lab, Boulder, CO USA. RP Biraud, SC (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM scbiraud@lbl.gov RI Biraud, Sebastien/M-5267-2013; Riley, William/D-3345-2015; Torn, Margaret/D-2305-2015 OI Biraud, Sebastien/0000-0001-7697-933X; Riley, William/0000-0002-4615-2304; FU Office of Biological and Environmental Research of the US Department of Energy [DE-AC02-05CH11231]; Office of Biological and Environmental Research of the US Department of Energy as part of the Atmospheric Radiation Measurement Program (ARM); Office of Biological and Environmental Research of the US Department of Energy as part of the ARM Aerial Facility; Office of Biological and Environmental Research of the US Department of Energy as part of the Terrestrial Ecosystem Science Program; SBIR from the US Department of Commerce; US Department of Energy; National Aeronautics and Space Administration FX This research was supported by the Office of Biological and Environmental Research of the US Department of Energy under contract No. DE-AC02-05CH11231 as part of the Atmospheric Radiation Measurement Program (ARM), ARM Aerial Facility, and Terrestrial Ecosystem Science Program. AOS was supported by SBIR grants over a ten year period from the US Department of Commerce, the US Department of Energy and the National Aeronautics and Space Administration. The authors thank their colleagues for continuing support and discussion during the coffee breaks; The Greenwood group and pilot Bob Fristoe for their dedication to the program. NR 52 TC 21 Z9 21 U1 4 U2 30 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1867-1381 J9 ATMOS MEAS TECH JI Atmos. Meas. Tech. PY 2013 VL 6 IS 3 BP 751 EP 763 DI 10.5194/amt-6-751-2013 PG 13 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 118GA UT WOS:000317011200018 ER PT S AU Velarde, MC Demaria, M Campisi, J AF Velarde, Michael C. Demaria, Marco Campisi, Judith BE Extermann, M TI Senescent Cells and Their Secretory Phenotype as Targets for Cancer Therapy SO CANCER AND AGING: FROM BENCH TO CLINICS SE Interdisciplinary Topics in Gerontology LA English DT Article; Book Chapter ID INFLAMMATORY CYTOKINE SECRETION; BENIGN PROSTATIC HYPERPLASIA; GENOME-WIDE ASSOCIATION; CELLULAR SENESCENCE; TUMOR SUPPRESSION; HUMAN FIBROBLASTS; DNA-DAMAGE; EPITHELIAL-CELLS; GENE-EXPRESSION; MUTANT P53 AB Cancer is a devastating disease that increases exponentially with age. Cancer arises from cells that proliferate in an unregulated manner, an attribute that is countered by cellular senescence. Cellular senescence is a potent tumor-suppressive process that halts the proliferation, essentially irreversibly, of cells at risk for malignant transformation. A number of anti-cancer drugs have emerged that induce tumor cells to undergo cellular senescence. However, although a senescence response can halt the proliferation of cancer cells, the presence of senescent cells in tissues has been associated with age-related diseases, including, ironically, late-life cancer. Thus, anti-cancer therapies that can induce senescence might also drive aging phenotypes and age-related pathology. The deleterious effects of senescent cells most likely derive from their senescence-associated secretory phenotype or SASP. The SASP entails the secretion of numerous inflammatory cytokines, growth factors and proteases that can render the tissue microenvironment favorable for tumor growth. Here, we discuss the beneficial and detrimental effects of inducing cellular senescence, and propose strategies for targeting senescent cells as a means to fight cancer. Copyright (C) 2013 S. Karger AG, Basel C1 [Velarde, Michael C.; Demaria, Marco; Campisi, Judith] Buck Inst Res Aging, Novato, CA 94945 USA. [Campisi, Judith] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Campisi, J (reprint author), Buck Inst Res Aging, 8001 Redwood Blvd, Novato, CA 94945 USA. EM jcampisi@lbl.gov OI Demaria, Marco/0000-0002-8429-4813 FU NCI NIH HHS [R21 CA170610]; NIA NIH HHS [P01 AG041122, R37 AG009909, P01 AG017242] NR 75 TC 34 Z9 34 U1 0 U2 15 PU KARGER PI BASEL PA POSTFACH, CH-4009 BASEL, SWITZERLAND SN 0074-1132 BN 978-3-318-02306-0 J9 INTERD TOP GERONTOL JI Interdiscipl.Top.Gerontol. PY 2013 VL 38 BP 17 EP 27 DI 10.1159/000343572 PG 11 WC Oncology; Geriatrics & Gerontology SC Oncology; Geriatrics & Gerontology GA BEI47 UT WOS:000316708400003 PM 23503512 ER PT S AU Dingus, B AF Dingus, Brenda BE Ormes, JF TI The Anisotropy of Multi-TeV Cosmic Rays SO CENTENARY SYMPOSIUM 2012: DISCOVERY OF COSMIC RAYS SE AIP Conference Proceedings LA English DT Proceedings Paper CT Centenary Symposium on Discovery of Cosmic Rays CY JUN 26-28, 2012 CL Univ Denver, Denver, CO SP Natl Sci Fdn (NSF), Univ Denver, Off Res and Sponsored Programs, Univ Denver, Div Nat Sci and Math, Univ Denver, Dept Phys and Astronomy, Stanford Univ, Kavli Inst Particle Astrophys and Cosmol (KIPAC) HO Univ Denver DE TeV Gamma-rays; Water Cherenkov ID GALACTIC PLANE; MILAGRO; EMISSION; REGION AB The arrival directions of cosmic rays will be isotropized by the deflection of these charged particles in the Galactic magnetic fields. For example, a 10 TeV proton in a typical Galactic field of 2 microGauss has a gyroradius of only 0.005 parsec (=1000 AU) which is much smaller than the distance to any postulated sources. However, observations of TeV cosmic rays by Milagro, Tibet III, ARGO, and IceCube, show anisotropies on both large and small angular scales. These observations require the detection of large numbers of cosmic rays because the anisotropies are less than a few parts in 1000. The large angular scale anisotropies, such as a dipole, could point to diffusion from a nearby source, but the smaller scale anisotropies of extent similar to 10 degrees are much more difficult to explain. Possibilities that have been explored in the literature include magnetic funneling of cosmic rays from nearby sources and acceleration by magnetic reconnection in the heliosphere's magnetotail. No matter what the mechanism, these observations provide new information about cosmic ray production, nearby magnetic fields, and how the cosmic rays observed at Earth are affected by their propagation. C1 Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Dingus, B (reprint author), Los Alamos Natl Lab, P-23 SM-30 Bikini Atoll Rd,MS H803, Los Alamos, NM 87545 USA. OI Dingus, Brenda/0000-0001-8451-7450 NR 8 TC 0 Z9 0 U1 0 U2 0 PU AMER INST PHYSICS PI MELVILLE PA 2 HUNTINGTON QUADRANGLE, STE 1NO1, MELVILLE, NY 11747-4501 USA SN 0094-243X BN 978-0-7354-1137-1 J9 AIP CONF PROC PY 2013 VL 1516 BP 254 EP 254 DI 10.1063/1.4792579 PG 1 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA BEH31 UT WOS:000316575600049 ER PT J AU Cholewa, PP Beavers, CM Teat, SJ Dalgarno, SJ AF Cholewa, Piotr P. Beavers, Christine M. Teat, Simon J. Dalgarno, Scott J. TI Directed assembly via selectively positioned host functionality SO CHEMICAL COMMUNICATIONS LA English DT Article ID METAL-ORGANIC FRAMEWORKS; POLYHEDRA; NANOTUBES; COMPLEXES; CHEMISTRY; RIM AB Introduction of distal carboxylic acid groups over two positions at the upper-rim of a di-O-alkylcalix[4]arene provides facile control over coordination polymer or discrete metal-organic capsule formation. C1 [Cholewa, Piotr P.; Dalgarno, Scott J.] Heriot Watt Univ, Inst Chem Sci, Edinburgh EH14 4AS, Midlothian, Scotland. [Beavers, Christine M.; Teat, Simon J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Dalgarno, SJ (reprint author), Heriot Watt Univ, Inst Chem Sci, Edinburgh EH14 4AS, Midlothian, Scotland. EM S.J.Dalgarno@hw.ac.uk RI Beavers, Christine/C-3539-2009; Dalgarno, Scott/A-7358-2010 OI Beavers, Christine/0000-0001-8653-5513; Dalgarno, Scott/0000-0001-7831-012X FU Office of Science, Office of Basic Energy Sciences, of the US Department of Energy [DE-AC02-05CH11231]; EPSRC FX The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the US Department of Energy under contract no. DE-AC02-05CH11231. We thank the EPSRC for financial support of this work. NR 24 TC 12 Z9 12 U1 0 U2 26 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1359-7345 J9 CHEM COMMUN JI Chem. Commun. PY 2013 VL 49 IS 31 BP 3203 EP 3205 DI 10.1039/c3cc40564h PG 3 WC Chemistry, Multidisciplinary SC Chemistry GA 112XD UT WOS:000316627000007 PM 23486785 ER PT J AU Peng, R Wu, CM Baltrusaitis, J Dimitrijevic, NM Rajh, T Koodali, RT AF Peng, Rui Wu, Chia-Ming Baltrusaitis, Jonas Dimitrijevic, Nada M. Rajh, Tijana Koodali, Ranjit T. TI Ultra-stable CdS incorporated Ti-MCM-48 mesoporous materials for efficient photocatalytic decomposition of water under visible light illumination SO CHEMICAL COMMUNICATIONS LA English DT Article ID HYDROGEN GENERATION; IRRADIATION; OXIDATION; CLEAVAGE; SYSTEMS AB A RuO2-CdS-Ti-MCM-48 mesoporous material has been prepared. This composite material generates hydrogen and oxygen in the absence of a Pt co-catalyst and most importantly photocorrosion of CdS is completely eliminated. C1 [Peng, Rui; Wu, Chia-Ming; Koodali, Ranjit T.] Univ S Dakota, Dept Chem, Vermillion, SD 57069 USA. [Baltrusaitis, Jonas] Univ Twente, PhotoCatalyt Synth Grp, Enschede, Netherlands. [Dimitrijevic, Nada M.; Rajh, Tijana] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Dimitrijevic, Nada M.; Rajh, Tijana] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Koodali, RT (reprint author), Univ S Dakota, Dept Chem, Vermillion, SD 57069 USA. EM Ranjit.Koodali@usd.edu RI Koodali, Ranjit/E-5595-2011; Baltrusaitis, Jonas/F-9367-2013; Peng, Rui/J-3781-2016; OI Koodali, Ranjit/0000-0002-2790-3053; Peng, Rui/0000-0002-1686-9574; Baltrusaitis, Jonas/0000-0001-5634-955X FU U.S. DOE [DE-AC02-06CH11357]; [NSF-CHE-0722632]; [NSF-EPS-0903804]; [DE-EE0000270]; [SD NASA-EPSCOR NNX12AB17G] FX Thanks are due to NSF-CHE-0722632, NSF-EPS-0903804, DE-EE0000270, and SD NASA-EPSCOR NNX12AB17G. The work at the Center for Nanoscale Materials was supported by the U.S. DOE, under contract DE-AC02-06CH11357. NR 23 TC 29 Z9 29 U1 4 U2 94 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1359-7345 J9 CHEM COMMUN JI Chem. Commun. PY 2013 VL 49 IS 31 BP 3221 EP 3223 DI 10.1039/c3cc41362d PG 3 WC Chemistry, Multidisciplinary SC Chemistry GA 112XD UT WOS:000316627000013 PM 23482963 ER PT J AU Wu, G More, KL Xu, P Wang, HL Ferrandon, M Kropf, AJ Myers, DJ Ma, SG Johnston, CM Zelenay, P AF Wu, Gang More, Karren L. Xu, Ping Wang, Hsing-Lin Ferrandon, Magali Kropf, Arthur J. Myers, Deborah J. Ma, Shuguo Johnston, Christina M. Zelenay, Piotr TI A carbon-nanotube-supported graphene-rich non-precious metal oxygen reduction catalyst with enhanced performance durability SO CHEMICAL COMMUNICATIONS LA English DT Article ID MEMBRANE FUEL-CELLS; POLYANILINE; IRON; ELECTROCATALYSTS; ELECTRODES; OXIDATION AB A non-precious metal catalyst for oxygen reduction in acid media, enriched in graphene sheets/bubbles during a high-temperature synthesis step, has been developed from an Fe precursor and in situ polymerized polyaniline, supported on multi-walled carbon nanotubes. The catalyst showed no performance loss for 500 hours in a hydrogen/air fuel cell. The improved durability is correlated with the graphene formation, apparently enhanced in the presence of carbon nanotubes. C1 [Wu, Gang; Johnston, Christina M.; Zelenay, Piotr] Mat Phys & Applicat Div, Los Alamos, NM 87545 USA. [More, Karren L.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Xu, Ping; Wang, Hsing-Lin] Los Alamos Natl Lab, Div Chem, Los Alamos, NM 87545 USA. [Ferrandon, Magali; Kropf, Arthur J.; Myers, Deborah J.] Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA. [Ma, Shuguo] Univ S Carolina, Dept Chem Engn, Columbia, SC 29208 USA. RP Wu, G (reprint author), Mat Phys & Applicat Div, Los Alamos, NM 87545 USA. EM wugang@lanl.gov; zelenay@lanl.gov RI Wu, Gang/E-8536-2010; Xu, Ping/I-1910-2013; More, Karren/A-8097-2016 OI Wu, Gang/0000-0003-4956-5208; Xu, Ping/0000-0002-1516-4986; More, Karren/0000-0001-5223-9097 FU U.S. DOE's Fuel Cell Technologies Program; LANL Laboratory-Directed Research and Development Programs; Office of Science; Office of Basic Energy Sciences; ORNL's ShaRE User Facility; Office of Basic Energy Sciences, U.S. DOE FX This research was supported by the U.S. DOE's Fuel Cell Technologies Program and LANL Laboratory-Directed Research and Development Programs. The use of the Advanced Photon Source at ANL was supported by the Office of Science, and the Office of Basic Energy Sciences. Microscopy research was supported by ORNL's ShaRE User Facility, sponsored by the Office of Basic Energy Sciences, U.S. DOE. NR 14 TC 88 Z9 88 U1 9 U2 226 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1359-7345 J9 CHEM COMMUN JI Chem. Commun. PY 2013 VL 49 IS 32 BP 3291 EP 3293 DI 10.1039/c3cc39121c PG 3 WC Chemistry, Multidisciplinary SC Chemistry GA 113TZ UT WOS:000316693100003 PM 23420477 ER PT J AU Akpinar, H Schlueter, JA Lahti, PM AF Akpinar, Handan Schlueter, John A. Lahti, Paul M. TI 2-(9,10-Anthraquinon-2-yl)-4,4,5,5-tetramethyl-4,5-dihydro-1H-imidazole- 3-oxide-1-oxyl: polymorphism in a conjugated anthraquinone-substituted nitronylnitroxide SO CHEMICAL COMMUNICATIONS LA English DT Article ID BOTTOM-UP; DENSITY; CRYSTAL AB Two polymorphs of an anthraquinone-nitronylnitroxide radical, AntQNN, were isolated, both with antiferromagnetic (AFM) exchange attributed to chain-type inter-radical contacts: one with J(1D)/k approximate to -3 K, and one with J(1D)/k approximate to -17 K. C1 [Akpinar, Handan; Lahti, Paul M.] Univ Massachusetts, Dept Chem, Amherst, MA 01003 USA. [Schlueter, John A.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Lahti, PM (reprint author), Univ Massachusetts, Dept Chem, Amherst, MA 01003 USA. EM jaschlueter@anl.gov; lahti@chem.umass.edu FU National Science Foundation [CHE-0809791]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; National Science Foundation/Department of Energy [NSF/CHE-0822838] FX This work (HA, PML) was supported by the National Science Foundation grant CHE-0809791. Use of the Advanced Photon Source (JAS) was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. ChemMatCARS Sector 15 is principally supported by the National Science Foundation/Department of Energy under grant number NSF/CHE-0822838. NR 17 TC 3 Z9 3 U1 0 U2 14 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1359-7345 J9 CHEM COMMUN JI Chem. Commun. PY 2013 VL 49 IS 32 BP 3345 EP 3347 DI 10.1039/c3cc41075g PG 3 WC Chemistry, Multidisciplinary SC Chemistry GA 113TZ UT WOS:000316693100021 PM 23503573 ER PT J AU Shen, ZL Kim, J Shen, JM Downing, CM Lee, S Kung, HH Kung, MC AF Shen, Zhongliang Kim, Jongsik Shen, Jingmei Downing, Christopher M. Lee, Sungsik Kung, Harold H. Kung, Mayfair C. TI Spherosilicates with peripheral malonic acid and vinyl end groups SO CHEMICAL COMMUNICATIONS LA English DT Article ID POLYHEDRAL OLIGOSILSESQUIOXANE; SILYL ESTERS; DENDRIMERS; SILSESQUIOXANES; PRECURSORS; NANOCAGES; LIQUID; ROUTE; CORE AB Two novel spherosilicates comprised of an octahedral Si8O12 core, [Si8O12]-(OSiMe2CH2CH2CH2CH(COOH)(2))(8) and [Si8O12]-(OSiMe2CH2CH2CH2CH(COOSi(CH=CH2)(3))(2))(8), were synthesized from [Si8O12]-(OSiMe2H)(8). These new structures have high densities of peripheral functional groups, and the second structure also possesses silyl ester bonds that are easily cleavable under mild conditions. These functionalities enable these structures to be modified further and to have many potential applications. We demonstrated one by cross-linking the vinyl-terminated spherosilicate to form nanospheres with a narrow size distribution and utilizing the hydrophilic interior to accommodate a Pd salt in a toluene solution. C1 [Shen, Zhongliang; Kim, Jongsik; Shen, Jingmei; Kung, Harold H.; Kung, Mayfair C.] Northwestern Univ, Dept Chem & Biol Engn, Evanston, IL 60208 USA. [Downing, Christopher M.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Lee, Sungsik] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. RP Kung, MC (reprint author), Northwestern Univ, Dept Chem & Biol Engn, 2145 Sheridan Rd, Evanston, IL 60208 USA. EM m-kung@northwestern.edu RI Kung, Harold/B-7647-2009; Kung, Mayfair/B-7648-2009 FU Institute for Atom-efficient Chemical Transformations (IACT), an Energy Frontier Research Center; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences FX This report is based on work supported as part of the Institute for Atom-efficient Chemical Transformations (IACT), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. We would also like to thank Andrea Luthi from Professor Chad Mirkin's group for assistance with DLS, and Archana Krovi from Professor SonBinh Nguyen's group for assistance with GPC. NR 33 TC 6 Z9 6 U1 2 U2 25 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1359-7345 J9 CHEM COMMUN JI Chem. Commun. PY 2013 VL 49 IS 32 BP 3357 EP 3359 DI 10.1039/c3cc40533h PG 3 WC Chemistry, Multidisciplinary SC Chemistry GA 113TZ UT WOS:000316693100025 PM 23503304 ER PT J AU Kang, LL Xu, P Zhang, B Tsai, HH Han, XJ Wang, HL AF Kang, Leilei Xu, Ping Zhang, Bin Tsai, Hsinhan Han, Xijiang Wang, Hsing-Lin TI Laser wavelength- and power-dependent plasmon-driven chemical reactions monitored using single particle surface enhanced Raman spectroscopy SO CHEMICAL COMMUNICATIONS LA English DT Article ID CATALYTIC-PROPERTIES; P-AMINOTHIOPHENOL; AU; NANOPARTICLES; AG; P,P'-DIMERCAPTOAZOBENZENE; MOLECULE; SCATTERING; JUNCTIONS AB Plasmon-driven chemical reaction of p-nitrothiophenol (pNTP) dimerizing into p,p'-dimercaptoazobenzene (DMAB) has been monitored using single particle surface enhanced Raman spectroscopy, which provides laser wavelength- and power-dependent conversion rates of the reaction. C1 [Kang, Leilei; Xu, Ping; Zhang, Bin; Han, Xijiang] Harbin Inst Technol, Dept Chem, Harbin 150001, Peoples R China. [Xu, Ping; Tsai, Hsinhan; Wang, Hsing-Lin] Los Alamos Natl Lab, Div Chem, Los Alamos, NM 87545 USA. RP Xu, P (reprint author), Harbin Inst Technol, Dept Chem, Harbin 150001, Peoples R China. EM pxu@hit.edu.cn; hanxj63@yahoo.com.cn; hwang@lanl.gov RI Xu, Ping/I-1910-2013 OI Xu, Ping/0000-0002-1516-4986 FU China Postdoctoral Fund; NSFC [21203045, 21101041, 21003029, 21071037, 91122002]; Fundamental Research Funds for the Central Universities [HIT.NSRIF. 2010065, 2011017, HIT.BRETIII. 201223]; LANL; Laboratory Directed Research and Development (LDRD) fund under DOE; Basic Energy Science (BES), Biomaterials program, Materials Sciences and Engineering Division FX PX thanks support from the China Postdoctoral Fund, NSFC (No. 21203045, 21101041, 21003029, 21071037, 91122002), Fundamental Research Funds for the Central Universities (No. HIT.NSRIF. 2010065 and 2011017, and HIT.BRETIII. 201223), and Director's Postdoctoral Fellow from LANL. HLW acknowledges the financial support from the Laboratory Directed Research and Development (LDRD) fund under the auspices of DOE. This work was partially supported by Basic Energy Science (BES), Biomaterials program, Materials Sciences and Engineering Division. NR 21 TC 58 Z9 58 U1 7 U2 135 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1359-7345 J9 CHEM COMMUN JI Chem. Commun. PY 2013 VL 49 IS 33 BP 3389 EP 3391 DI 10.1039/c3cc40732b PG 3 WC Chemistry, Multidisciplinary SC Chemistry GA 117MW UT WOS:000316958600002 PM 23440353 ER PT J AU Tian, CC Chai, SH Mullins, DR Zhu, X Binder, A Guo, YL Dai, S AF Tian, Chengcheng Chai, Song-Hai Mullins, David R. Zhu, Xiang Binder, Andrew Guo, Yanglong Dai, Sheng TI Heterostructured BaSO4-SiO2 mesoporous materials as new supports for gold nanoparticles in low-temperature CO oxidation SO CHEMICAL COMMUNICATIONS LA English DT Article ID AU CATALYSTS; CLUSTERS; TITANIA AB Nanosized BaSO4-based mesoporous hybrid materials have been developed and identified as new efficient inorganic salt-based support systems for ultrastable gold nanoparticles in low-temperature CO oxidation. C1 [Tian, Chengcheng; Zhu, Xiang; Guo, Yanglong] E China Univ Sci & Technol, Res Inst Ind Catalysis, Key Lab Adv Mat, Shanghai 200237, Peoples R China. [Tian, Chengcheng; Chai, Song-Hai; Mullins, David R.; Zhu, Xiang; Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Binder, Andrew; Dai, Sheng] Univ Tennessee, Dept Chem, Knoxville, TN 37916 USA. RP Chai, SH (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. EM chais@ornl.gov; ylguo@ecust.edu.cn; dais@ornl.gov RI Chai, Song-Hai/A-9299-2012; Zhu, Xiang/P-6867-2014; Dai, Sheng/K-8411-2015 OI Chai, Song-Hai/0000-0002-4152-2513; Zhu, Xiang/0000-0002-3973-4998; Dai, Sheng/0000-0002-8046-3931 FU Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, US Department of Energy FX We would like to acknowledge the financial support from the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, US Department of Energy. CCT and YLG also thank National Basic Research Program of China. NR 19 TC 7 Z9 8 U1 8 U2 87 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1359-7345 J9 CHEM COMMUN JI Chem. Commun. PY 2013 VL 49 IS 33 BP 3464 EP 3466 DI 10.1039/c3cc41167b PG 3 WC Chemistry, Multidisciplinary SC Chemistry GA 117MW UT WOS:000316958600027 PM 23511903 ER PT J AU Lapidus, SH Manson, JL Liu, JJ Smith, MJ Goddard, P Bendix, J Topping, CV Singleton, J Dunmars, C Mitchell, JF Schlueter, JA AF Lapidus, Saul H. Manson, Jamie L. Liu, Junjie Smith, Matthew J. Goddard, Paul Bendix, Jesper Topping, Craig V. Singleton, John Dunmars, Cortney Mitchell, J. F. Schlueter, John A. TI Quantifying magnetic exchange in doubly-bridged Cu-X-2-Cu (X = F, Cl, Br) chains enabled by solid state synthesis of CuF2(pyrazine) SO CHEMICAL COMMUNICATIONS LA English DT Article ID POWDER DIFFRACTION DATA; CRYSTAL; COMPLEXES; PYRAZINE; PRESSURE; ZIGZAG AB Solid state techniques involving pressure and temperature have been used to synthesize the fluoride member of the CuX2(pyrazine) (X = F, Cl, Br) family of coordination polymers that cannot be crystallized by solution methods. CuF2(pyrazine) exhibits unique trans doubly-bridged Cu-F-2-Cu chains that provide an opportunity to quantify magnetic superexchange in an isostructural Cu-X-2-Cu series. C1 [Lapidus, Saul H.; Dunmars, Cortney; Mitchell, J. F.; Schlueter, John A.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Manson, Jamie L.] Eastern Washington Univ, Dept Chem & Biochem, Cheney, WA 99004 USA. [Liu, Junjie; Smith, Matthew J.; Goddard, Paul] Univ Oxford, Dept Phys, Clarendon Lab, Oxford OX1 3PU, England. [Bendix, Jesper] Univ Copenhagen, Dept Chem, DK-2100 Copenhagen, Denmark. [Topping, Craig V.; Singleton, John] Los Alamos Natl Lab, Natl High Magnet Field Lab, Los Alamos, NM 87545 USA. RP Schlueter, JA (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM JASchlueter@anl.gov RI Liu, Junjie/B-1643-2013; Goddard, Paul/A-8638-2015; Bendix, Jesper/H-5468-2012 OI Goddard, Paul/0000-0002-0666-5236; Bendix, Jesper/0000-0003-1255-2868 FU UChicago Argonne, LLC; U.S. Department of Energy Office of Science laboratory [DE-AC02-06CH11357]; U.S. National Science Foundation [DMR-1005825]; NSF [DMR-0654118]; State of Florida; U.S. DoE BES program "Science in 100 T"; EPSRC FX We thank S. Brombosz for technical assistance. Work at ANL, including the APS, was supported by UChicago Argonne, LLC, Operator of Argonne National Laboratory ("Argonne"). Argonne, a U.S. Department of Energy Office of Science laboratory, is operated under Contract No. DE-AC02-06CH11357. Work at EWU was supported by the U.S. National Science Foundation under Grant No. DMR-1005825. Work performed at the NHMFL was supported by the NSF Cooperative Agreement No. DMR-0654118, the State of Florida, and the U.S. DoE BES program "Science in 100 T." Work in the UK was supported by EPSRC. NR 21 TC 6 Z9 6 U1 2 U2 41 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1359-7345 J9 CHEM COMMUN JI Chem. Commun. PY 2013 VL 49 IS 34 BP 3558 EP 3560 DI 10.1039/c3cc41394b PG 3 WC Chemistry, Multidisciplinary SC Chemistry GA 117NT UT WOS:000316960900018 PM 23525300 ER PT J AU Geier, SJ Mason, JA Bloch, ED Queen, WL Hudson, MR Brown, CM Long, JR AF Geier, Stephen J. Mason, Jarad A. Bloch, Eric D. Queen, Wendy L. Hudson, Matthew R. Brown, Craig M. Long, Jeffrey R. TI Selective adsorption of ethylene over ethane and propylene over propane in the metal-organic frameworks M-2(dobdc) (M = Mg, Mn, Fe, Co, Ni, Zn) SO CHEMICAL SCIENCE LA English DT Article ID CARBON-DIOXIDE CAPTURE; IRON(II) COORDINATION SITES; HYDROGEN STORAGE; KINETIC SEPARATION; OLEFIN/PARAFFIN SEPARATIONS; ROOM-TEMPERATURE; METHANE STORAGE; HIGH-CAPACITY; COMPLEXES; ACETYLENE AB A significant reduction in the energy costs associated with the cryogenic separation of ethylene-ethane and propylene-propane mixtures could potentially be realized through the use of selective solid adsorbents that operate at higher temperatures. The metal-organic frameworks M-2(dobdc) (M = Mg, Mn, Fe, Co, Ni, Zn; dobdc(4-) = 2,5-dioxido-1,4-benzenedicarboxylate) are of particular interest for this application, owing to their high density of coordinatively unsaturated M2+ cation sites that can selectively interact with unsaturated hydrocarbons. Here, we present gas adsorption data for ethylene, ethane, propylene, and propane at 45, 60, and 80 degrees C for the entire series. The means of sample preparation and activation is found to be important for achieving high separation selectivities and capacities. While all of the compounds investigated show good performance characteristics, Fe-2(dobdc) and Mn-2(dobdc) exhibit the highest selectivities for the separation of ethylene-ethane and propylene-propane mixtures, respectively. Crystal structures determined from neutron powder diffraction data elucidate the binding of ethane, ethylene, and propylene in Mn2(dobdc) and Co-2(dobdc). C1 [Geier, Stephen J.; Mason, Jarad A.; Bloch, Eric D.; Long, Jeffrey R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Queen, Wendy L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Queen, Wendy L.; Hudson, Matthew R.; Brown, Craig M.] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Brown, Craig M.] Univ Delaware, Dept Chem Engn, Newark, DE 19716 USA. [Long, Jeffrey R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Long, JR (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM jrlong@berkeley.edu RI EFRC, CGS/I-6680-2012; Stangl, Kristin/D-1502-2015; Brown, Craig/B-5430-2009; Foundry, Molecular/G-9968-2014; OI Brown, Craig/0000-0002-9637-9355; Queen, Wendy/0000-0002-8375-2341 FU Center for Gas Separations Relevant to Clean Energy Technologies, an Energy Frontier Research Center; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001015]; Camille and Henry Dreyfus Foundation; NSERC; National Science Foundation; NIST/NRC FX This research was funded through the Center for Gas Separations Relevant to Clean Energy Technologies, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award no. DE-SC0001015. We thank the Camille and Henry Dreyfus Foundation Postdoctoral Program in Environmental Chemistry and NSERC for support of S. J. G., the National Science Foundation for fellowship support of J. A. M, and support for W. L. Q. and M. R. H. from the NIST/NRC Fellowship Program. NR 80 TC 110 Z9 111 U1 15 U2 202 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2041-6520 EI 2041-6539 J9 CHEM SCI JI Chem. Sci. PY 2013 VL 4 IS 5 BP 2054 EP 2061 DI 10.1039/c3sc00032j PG 8 WC Chemistry, Multidisciplinary SC Chemistry GA 117PV UT WOS:000316966500015 ER PT J AU Bakac, A Pestovsky, O Durfey, BL Kristian, KE AF Bakac, Andreja Pestovsky, Oleg Durfey, Bridget L. Kristian, Kathleen E. TI Kinetics and thermodynamics of nitric oxide binding to transition metal complexes. Relationship to dioxygen binding SO CHEMICAL SCIENCE LA English DT Article ID OXIDATION-REDUCTION REACTIONS; ELECTRON-TRANSFER REACTIONS; REVERSIBLE BINDING; MOLECULAR-OXYGEN; NITROUS-ACID; SUPEROXORHODIUM(III) COMPLEX; SUPEROXOCHROMIUM(III) ION; COORDINATION CHEMISTRY; MACROCYCLIC LIGANDS; AQUEOUS-SOLUTIONS AB The kinetics and activation parameters for NO dissociation from L(H2O)Co(NO)(2+) (L = L-1 = cyclam and L-2 = meso-Me-6-cyclam), L-2(H2O)Rh(NO)(2+), and Cr(H2O)(5)NO2+ were determined in aqueous solution in the presence of IrCl62, IrBr62, or O-2 as scavengers for NO and/or metal(II) complexes. The rate constants k(-NO) at 25 degrees C are (5.7 +/- 0.1) x 10(-3) s(-1) for L-2(H2O)Co(NO)(2+), (1.0 +/- 0.1) x 10(-4) for L-1(H2O)Co(NO)(2+), (5.9 +/- 2.0) x 10(-8) for Cr(H2O)(5)NO2+ and (3.5 +/- 1.8) x 10(-9) s(-1) for L-2(H2O)Rh(NO)(2+). The kinetics of the reverse reaction were determined by laser flash photolysis at 25 degrees C, k(NO) = (1.7 +/- 0.2) x 10(7) M-1 s(-1) for (LCo)-Co-2(H2O)(2)(2+) and (1.8 +/- 0.1) x 10(8) M-1 s(-1) for L-2(H2O)Rh2+. The rate constants k(NO) and k(-NO) obtained here and those available in the literature were used to calculate the equilibrium binding constants K-NO for a series of nitrosyl metal complexes. A good correlation was found between log K-NO and log K-O2, the latter corresponding to O-2 binding. The correlation includes complexes of four different transition metals as well as hydrogen atom, and covers a range of about 3 V in reduction potentials. The implications of these results are discussed. C1 [Bakac, Andreja; Durfey, Bridget L.; Kristian, Kathleen E.] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. [Bakac, Andreja; Pestovsky, Oleg] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. RP Bakac, A (reprint author), Iowa State Univ, Dept Chem, Ames, IA 50011 USA. EM bakac@ameslab.gov FU National Science Foundation [CHE 0602183]; U.S. Department of Energy, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division through the Ames Laboratory; U.S. Department of Energy by Iowa State University [DE-AC02-07CH11358] FX This research was supported by Award no. CHE 0602183 to AB from the National Science Foundation (B.L.D., K.E.K) and the U.S. Department of Energy, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division through the Ames Laboratory (A.B., O. P.). The Ames Laboratory is operated for the U.S. Department of Energy by Iowa State University under Contract no. DE-AC02-07CH11358. NR 76 TC 2 Z9 2 U1 1 U2 23 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2041-6520 J9 CHEM SCI JI Chem. Sci. PY 2013 VL 4 IS 5 BP 2185 EP 2192 DI 10.1039/c3sc50157d PG 8 WC Chemistry, Multidisciplinary SC Chemistry GA 117PV UT WOS:000316966500033 ER PT J AU Cordones, AA Leone, SR AF Cordones, Amy A. Leone, Stephen R. TI Mechanisms for charge trapping in single semiconductor nanocrystals probed by fluorescence blinking SO CHEMICAL SOCIETY REVIEWS LA English DT Review ID QUANTUM-DOT BLINKING; POWER-LAW BEHAVIOR; CDSE NANOCRYSTALS; RATE FLUCTUATIONS; SURFACE TRAPS; INTERMITTENCY; SPECTROSCOPY; DYNAMICS; STATISTICS; DEPENDENCE AB Semiconductor nanocrystal optical and charge transport properties are largely influenced by the trapping of charge carriers on the nanocrystal surface. Charge trapping increases the non-radiative exciton decay pathways, thus decreasing the fluorescence quantum yield, and it also impedes efficient charge transfer at the nanocrystal interface. On a single nanocrystal basis, charge trapping causes interruptions in the otherwise continuous fluorescence known as fluorescence intermittency or blinking. In this tutorial review we examine the relationship between charge trapping and fluorescence blinking. The fluorescence microscopy techniques and statistical analysis methods used to measure single nanocrystal blinking are introduced. The development of numerous blinking mechanisms is reviewed, as is the physical nature of charge trapping sites. An overview of blinking experiments used to probe specific mechanisms for charge carrier trapping is presented. Finally, a summary and outlook are offered. Although the detailed mechanism is not fully understood, blinking experiments are found to provide direct evidence for several charge trapping mechanisms and report on changes to the nature and distribution of charge trapping sites. C1 [Leone, Stephen R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Leone, SR (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM srl@berkeley.edu FU program Physical Chemistry of Inorganic Nanostructures by Office of Science, Office of Basic Energy Sciences, U.S. Department of Energy through the Materials Research Division [KC3103, DE-AC02-05CH11231] FX This work was supported by the program Physical Chemistry of Inorganic Nanostructures, KC3103, which is supported by the Director, Office of Science, Office of Basic Energy Sciences, U.S. Department of Energy under Contract No. DE-AC02-05CH11231 through the Materials Research Division. NR 54 TC 33 Z9 33 U1 3 U2 78 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 0306-0012 J9 CHEM SOC REV JI Chem. Soc. Rev. PY 2013 VL 42 IS 8 BP 3209 EP 3221 DI 10.1039/c2cs35452g PG 13 WC Chemistry, Multidisciplinary SC Chemistry GA 116FZ UT WOS:000316869700003 PM 23306775 ER PT J AU Tian, GX Teat, SJ Rao, LF AF Tian, Guoxin Teat, Simon J. Rao, Linfeng TI Thermodynamic studies of U(VI) complexation with glutardiamidoxime for sequestration of uranium from seawater SO DALTON TRANSACTIONS LA English DT Article ID SEA-WATER; EQUILIBRIUM-CONSTANTS; EXTRACTION; AMIDOXIMES; RECOVERY; SORBERS AB Glutardiamidoxime (H2B), a diamidoxime ligand that has implications in sequestering uranium from seawater, forms strong complexes with UO22+. Five U(VI) complexes were identified in 3% NaCl solution. The stability constants and the enthalpies of complexation were measured by potentiometry and microcalorimetry. The competition between glutardiamidoxime and carbonate for complexing U(VI) in 3% NaCl was also studied in comparison with the cyclic glutarimidedioxime ligand (H(2)A) previously studied. C1 [Tian, Guoxin; Rao, Linfeng] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Teat, Simon J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Rao, LF (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM lrao@lbl.gov FU Uranium Resources Program, Fuel Cycle Research and Development Program, Office of Nuclear Energy of the U.S. Department of Energy (DOE) at Lawrence Berkeley National Laboratory (LBNL) [DE-AC02-05CH11231]; Office of Science, Office of Basic Energy Sciences, U.S. DOE [DE-AC02-05CH11231] FX This work was supported by the Uranium Resources Program, Fuel Cycle Research and Development Program, Office of Nuclear Energy of the U.S. Department of Energy (DOE) under Contract No. DE-AC02-05CH11231 at Lawrence Berkeley National Laboratory (LBNL). Single-crystal X-ray diffraction data were collected and analyzed at the Advanced Light Source (ALS). ALS is supported by the Director, Office of Science, Office of Basic Energy Sciences, U.S. DOE under Contract No. DE-AC02-05CH11231. NR 23 TC 27 Z9 28 U1 8 U2 66 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1477-9226 J9 DALTON T JI Dalton Trans. PY 2013 VL 42 IS 16 BP 5690 EP 5696 DI 10.1039/c3dt32940b PG 7 WC Chemistry, Inorganic & Nuclear SC Chemistry GA 116FW UT WOS:000316869400015 PM 23443817 ER PT S AU Ari-Gur, P Garlea, VO Coke, A Ge, YL Aaltio, I Hannula, SP Cao, HB Madiligama, ASB Koledov, V AF Ari-Gur, Pnina Garlea, V. Ovidiu Coke, Ashley Ge, Yanling Aaltio, Ilkka Hannula, Simo-Pekka Cao, Huibo Madiligama, Amila S. B. Koledov, Victor BE Prokoshkin, S Resnina, N TI NEUTRON DIFFRACTION STUDY OF A NON-STOICHIOMETRIC NI-Mn-Ga MSM ALLOY SO EUROPEAN SYMPOSIUM ON MARTENSITIC TRANSFORMATIONS SE Materials Science Forum LA English DT Proceedings Paper CT 9th European Symposium on Martensitic Transformations (ESOMAT 2012) CY SEP 09-16, 2012 CL St Petersburg, RUSSIA SP ANALIT ltd, Shimadzu Europa GmbH, Shimadzu Moscow Representat Off, Pruftechnik MT GMbH, ATM GMbH, Moscow Representat Off, Zwick GMbH & Co, St Petersburg Representat Off, BUEHLER, St Petersburg Representat Off, INSTRON, St Petersburg Representat Off, St Petersburg State Univ, Natl Univ Sci & Technol, Ioffe Phys Techn Inst RAS, Inst Metal Phys, Ural Branch RAS, Tomsk State Univ, Inst Radio Engn & Elect RAS, Natl Res Nucl Univ MEPhI, Inst Strength Phys & Mat Sci RAS, Ural State Forest Engn Univ, Chelyabinsk State Univ, Alpha Technologies, Kurdyumov Inst Met Phys DE Chemical Order; Ni-Mn-Ga alloy; Magnetic Shape Memory; Neutron Diffraction; Rietveld Method; Structure Refinement ID SINGLE-CRYSTALS; NI2MNGA; POWDER AB The structure and chemical order of a Heusler alloy of non-stoichiometric composition Ni-Mn-Ga were studied using constant-wavelength (1.538 angstrom) neutron difftaction at 363K and the diffraction pattern was refined using the FullProf software. At this temperature the structure is austenite (cubic) with Fm-3m space group and lattice constant of a = 5.83913(4) [angstrom]. The chemical order is of critical importance in these alloys, as Mn becomes antiferromagnetic when the atoms are closer than the radius of the 3d shell. In the studied alloy the refinement of the site occupancy showed that the 4h (Ga site) contained as much as 22% Mn; that significantly alters the distances between the Mn atoms in the crystal and, as a result, also the exchange energy between some of the Mn atoms. Based on the refinement, the composition was determined to be Ni1.91Mn1.29Ga0.8 C1 [Ari-Gur, Pnina; Madiligama, Amila S. B.] Western Michigan Univ, Kalamazoo, MI 49008 USA. [Garlea, V. Ovidiu; Coke, Ashley; Cao, Huibo] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Ge, Yanling; Aaltio, Ilkka; Hannula, Simo-Pekka] Aalto Univ Sch Chem Technol, Dept Mat Sci & Engn, Espoo, Finland. [Koledov, Victor] Russian Acad Sci, Moscow, Russia. RP Ari-Gur, P (reprint author), Western Michigan Univ, Kalamazoo, MI 49008 USA. EM pnina.ari-gur@wmich.edu; bgarleao@ornl.gov; yanling.ge@aalto.fi; ilkka.aaltio@aalto.fi; caoh@ornl.gov; gamila.bandara@wmich.edu; victor_koledov@mail.ru RI Aaltio, Ilkka/C-6170-2008; Victor, Koledov/F-4259-2014; Hannula, Simo-Pekka/G-2889-2012; Garlea, Vasile/A-4994-2016; Cao, Huibo/A-6835-2016 OI Aaltio, Ilkka/0000-0002-8759-0693; Hannula, Simo-Pekka/0000-0001-6247-0727; Garlea, Vasile/0000-0002-5322-7271; Cao, Huibo/0000-0002-5970-4980 NR 6 TC 1 Z9 1 U1 1 U2 7 PU TRANS TECH PUBLICATIONS LTD PI DURNTEN-ZURICH PA KREUZSTRASSE 10, 8635 DURNTEN-ZURICH, SWITZERLAND SN 0255-5476 J9 MATER SCI FORUM PY 2013 VL 738-739 BP 103 EP + DI 10.4028/www.scientific.net/MSF.738-739.103 PG 2 WC Materials Science, Multidisciplinary SC Materials Science GA BEC75 UT WOS:000316089000018 ER PT J AU Prager, S AF Prager, Stewart BA McCracken, G Stott, P BF McCracken, G Stott, P TI What Is Nuclear Fusion? SO FUSION: THE ENERGY OF THE UNIVERSE, 2ND EDITION LA English DT Article; Book Chapter C1 [Prager, Stewart] Univ Wisconsin, Madison, WI 53706 USA. [Prager, Stewart] US DOE, Fus Energy Sci Advisory Comm, Washington, DC 20585 USA. [Prager, Stewart] APS, Div Plasma Phys, Salt Lake City, UT USA. RP Prager, S (reprint author), Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08544 USA. NR 0 TC 0 Z9 0 U1 2 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA SARA BURGERHARTSTRAAT 25, PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS BN 978-0-08-049271-1 PY 2013 BP 1 EP 5 PG 5 WC Nuclear Science & Technology SC Nuclear Science & Technology GA BEI83 UT WOS:000316751600004 ER PT J AU Prager, S AF Prager, Stewart BA McCracken, G Stott, P BF McCracken, G Stott, P TI Energy from Mass SO FUSION: THE ENERGY OF THE UNIVERSE, 2ND EDITION LA English DT Article; Book Chapter C1 [Prager, Stewart] Univ Wisconsin, Madison, WI 53706 USA. [Prager, Stewart] US DOE, Fus Energy Sci Advisory Comm, Washington, DC 20585 USA. [Prager, Stewart] APS, Div Plasma Phys, Salt Lake City, UT USA. RP Prager, S (reprint author), Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08544 USA. NR 0 TC 0 Z9 0 U1 0 U2 1 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA SARA BURGERHARTSTRAAT 25, PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS BN 978-0-08-049271-1 PY 2013 BP 7 EP 14 PG 8 WC Nuclear Science & Technology SC Nuclear Science & Technology GA BEI83 UT WOS:000316751600005 ER PT J AU Prager, S AF Prager, Stewart BA McCracken, G Stott, P BF McCracken, G Stott, P TI Fusion The Energy of the Universe Second Edition Foreword to the Second Edition SO FUSION: THE ENERGY OF THE UNIVERSE, 2ND EDITION LA English DT Editorial Material; Book Chapter C1 [Prager, Stewart] Univ Wisconsin, Madison, WI 53706 USA. [Prager, Stewart] US DOE, Fus Energy Sci Advisory Comm, Washington, DC 20585 USA. [Prager, Stewart] APS, Div Plasma Phys, Salt Lake City, UT USA. RP Prager, S (reprint author), Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08544 USA. NR 0 TC 0 Z9 0 U1 2 U2 3 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA SARA BURGERHARTSTRAAT 25, PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS BN 978-0-08-049271-1 PY 2013 BP XIII EP XIV PG 2 WC Nuclear Science & Technology SC Nuclear Science & Technology GA BEI83 UT WOS:000316751600001 ER PT J AU Prager, S AF Prager, Stewart BA McCracken, G Stott, P BF McCracken, G Stott, P TI Fusion in the Sun and Stars SO FUSION: THE ENERGY OF THE UNIVERSE, 2ND EDITION LA English DT Article; Book Chapter C1 [Prager, Stewart] Univ Wisconsin, Madison, WI 53706 USA. [Prager, Stewart] US DOE, Fus Energy Sci Advisory Comm, Washington, DC 20585 USA. [Prager, Stewart] APS, Div Plasma Phys, Salt Lake City, UT USA. RP Prager, S (reprint author), Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08544 USA. NR 0 TC 0 Z9 0 U1 2 U2 3 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA SARA BURGERHARTSTRAAT 25, PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS BN 978-0-08-049271-1 PY 2013 BP 15 EP 29 PG 15 WC Nuclear Science & Technology SC Nuclear Science & Technology GA BEI83 UT WOS:000316751600006 ER PT B AU Prager, S AF Prager, Stewart BA McCracken, G Stott, P BF McCracken, G Stott, P TI Fusion The Energy of the Universe Second Edition Foreword to the First Edition SO FUSION: THE ENERGY OF THE UNIVERSE, 2ND EDITION LA English DT Editorial Material; Book Chapter C1 [Prager, Stewart] Univ Wisconsin, Madison, WI 53706 USA. [Prager, Stewart] US DOE, Fus Energy Sci Advisory Comm, Washington, DC 20585 USA. [Prager, Stewart] APS, Div Plasma Phys, Salt Lake City, UT USA. RP Prager, S (reprint author), Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08544 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA SARA BURGERHARTSTRAAT 25, PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS BN 978-0-08-049271-1 PY 2013 BP XV EP XVI PG 2 WC Nuclear Science & Technology SC Nuclear Science & Technology GA BEI83 UT WOS:000316751600002 ER PT B AU Prager, S AF Prager, Stewart BA McCracken, G Stott, P BF McCracken, G Stott, P TI Fusion The Energy of the Universe Second Edition Preface SO FUSION: THE ENERGY OF THE UNIVERSE, 2ND EDITION LA English DT Editorial Material; Book Chapter C1 [Prager, Stewart] Univ Wisconsin, Madison, WI 53706 USA. [Prager, Stewart] US DOE, Fus Energy Sci Advisory Comm, Washington, DC 20585 USA. [Prager, Stewart] APS, Div Plasma Phys, Salt Lake City, UT USA. RP Prager, S (reprint author), Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08544 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA SARA BURGERHARTSTRAAT 25, PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS BN 978-0-08-049271-1 PY 2013 BP XVII EP + PG 5 WC Nuclear Science & Technology SC Nuclear Science & Technology GA BEI83 UT WOS:000316751600003 ER PT B AU Prager, S AF Prager, Stewart BA McCracken, G Stott, P BF McCracken, G Stott, P TI Man-Made Fusion SO FUSION: THE ENERGY OF THE UNIVERSE, 2ND EDITION LA English DT Article; Book Chapter C1 [Prager, Stewart] Univ Wisconsin, Madison, WI 53706 USA. [Prager, Stewart] US DOE, Fus Energy Sci Advisory Comm, Washington, DC 20585 USA. [Prager, Stewart] APS, Div Plasma Phys, Salt Lake City, UT USA. RP Prager, S (reprint author), Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08544 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA SARA BURGERHARTSTRAAT 25, PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS BN 978-0-08-049271-1 PY 2013 BP 31 EP 43 PG 13 WC Nuclear Science & Technology SC Nuclear Science & Technology GA BEI83 UT WOS:000316751600007 ER PT B AU Prager, S AF Prager, Stewart BA McCracken, G Stott, P BF McCracken, G Stott, P TI Magnetic Confinement SO FUSION: THE ENERGY OF THE UNIVERSE, 2ND EDITION LA English DT Article; Book Chapter C1 [Prager, Stewart] Univ Wisconsin, Madison, WI 53706 USA. [Prager, Stewart] US DOE, Fus Energy Sci Advisory Comm, Washington, DC 20585 USA. [Prager, Stewart] APS, Div Plasma Phys, Salt Lake City, UT USA. RP Prager, S (reprint author), Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08544 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA SARA BURGERHARTSTRAAT 25, PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS BN 978-0-08-049271-1 PY 2013 BP 45 EP 58 PG 14 WC Nuclear Science & Technology SC Nuclear Science & Technology GA BEI83 UT WOS:000316751600008 ER PT J AU Prager, S AF Prager, Stewart BA McCracken, G Stott, P BF McCracken, G Stott, P TI The Hydrogen Bomb SO FUSION: THE ENERGY OF THE UNIVERSE, 2ND EDITION LA English DT Article; Book Chapter C1 [Prager, Stewart] Univ Wisconsin, Madison, WI 53706 USA. [Prager, Stewart] US DOE, Fus Energy Sci Advisory Comm, Washington, DC 20585 USA. [Prager, Stewart] APS, Div Plasma Phys, Salt Lake City, UT USA. RP Prager, S (reprint author), Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08544 USA. NR 0 TC 0 Z9 0 U1 1 U2 2 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA SARA BURGERHARTSTRAAT 25, PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS BN 978-0-08-049271-1 PY 2013 BP 59 EP 66 PG 8 WC Nuclear Science & Technology SC Nuclear Science & Technology GA BEI83 UT WOS:000316751600009 ER PT B AU Prager, S AF Prager, Stewart BA McCracken, G Stott, P BF McCracken, G Stott, P TI Inertial-Confinement Fusion SO FUSION: THE ENERGY OF THE UNIVERSE, 2ND EDITION LA English DT Article; Book Chapter C1 [Prager, Stewart] Univ Wisconsin, Madison, WI 53706 USA. [Prager, Stewart] US DOE, Fus Energy Sci Advisory Comm, Washington, DC 20585 USA. [Prager, Stewart] APS, Div Plasma Phys, Salt Lake City, UT USA. RP Prager, S (reprint author), Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08544 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA SARA BURGERHARTSTRAAT 25, PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS BN 978-0-08-049271-1 PY 2013 BP 67 EP 81 PG 15 WC Nuclear Science & Technology SC Nuclear Science & Technology GA BEI83 UT WOS:000316751600010 ER PT B AU Prager, S AF Prager, Stewart BA McCracken, G Stott, P BF McCracken, G Stott, P TI False Trails SO FUSION: THE ENERGY OF THE UNIVERSE, 2ND EDITION LA English DT Article; Book Chapter C1 [Prager, Stewart] Univ Wisconsin, Madison, WI 53706 USA. [Prager, Stewart] US DOE, Fus Energy Sci Advisory Comm, Washington, DC 20585 USA. [Prager, Stewart] APS, Div Plasma Phys, Salt Lake City, UT USA. RP Prager, S (reprint author), Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08544 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA SARA BURGERHARTSTRAAT 25, PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS BN 978-0-08-049271-1 PY 2013 BP 83 EP 90 PG 8 WC Nuclear Science & Technology SC Nuclear Science & Technology GA BEI83 UT WOS:000316751600011 ER PT B AU Prager, S AF Prager, Stewart BA McCracken, G Stott, P BF McCracken, G Stott, P TI Tokamaks SO FUSION: THE ENERGY OF THE UNIVERSE, 2ND EDITION LA English DT Article; Book Chapter C1 [Prager, Stewart] Univ Wisconsin, Madison, WI 53706 USA. [Prager, Stewart] US DOE, Fus Energy Sci Advisory Comm, Washington, DC 20585 USA. [Prager, Stewart] APS, Div Plasma Phys, Salt Lake City, UT USA. RP Prager, S (reprint author), Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08544 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA SARA BURGERHARTSTRAAT 25, PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS BN 978-0-08-049271-1 PY 2013 BP 91 EP 105 PG 15 WC Nuclear Science & Technology SC Nuclear Science & Technology GA BEI83 UT WOS:000316751600012 ER PT B AU Prager, S AF Prager, Stewart BA McCracken, G Stott, P BF McCracken, G Stott, P TI From T3 to ITER SO FUSION: THE ENERGY OF THE UNIVERSE, 2ND EDITION LA English DT Article; Book Chapter C1 [Prager, Stewart] Univ Wisconsin, Madison, WI 53706 USA. [Prager, Stewart] US DOE, Fus Energy Sci Advisory Comm, Washington, DC 20585 USA. [Prager, Stewart] APS, Div Plasma Phys, Salt Lake City, UT USA. RP Prager, S (reprint author), Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08544 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA SARA BURGERHARTSTRAAT 25, PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS BN 978-0-08-049271-1 PY 2013 BP 107 EP 127 PG 21 WC Nuclear Science & Technology SC Nuclear Science & Technology GA BEI83 UT WOS:000316751600013 ER PT B AU Prager, S AF Prager, Stewart BA McCracken, G Stott, P BF McCracken, G Stott, P TI ITER SO FUSION: THE ENERGY OF THE UNIVERSE, 2ND EDITION LA English DT Article; Book Chapter C1 [Prager, Stewart] Univ Wisconsin, Madison, WI 53706 USA. [Prager, Stewart] US DOE, Fus Energy Sci Advisory Comm, Washington, DC 20585 USA. [Prager, Stewart] APS, Div Plasma Phys, Salt Lake City, UT USA. RP Prager, S (reprint author), Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08544 USA. NR 0 TC 0 Z9 0 U1 1 U2 1 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA SARA BURGERHARTSTRAAT 25, PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS BN 978-0-08-049271-1 PY 2013 BP 129 EP 148 PG 20 WC Nuclear Science & Technology SC Nuclear Science & Technology GA BEI83 UT WOS:000316751600014 ER PT B AU Prager, S AF Prager, Stewart BA McCracken, G Stott, P BF McCracken, G Stott, P TI Large Inertial-Confinement Systems SO FUSION: THE ENERGY OF THE UNIVERSE, 2ND EDITION LA English DT Article; Book Chapter C1 [Prager, Stewart] Univ Wisconsin, Madison, WI 53706 USA. [Prager, Stewart] US DOE, Fus Energy Sci Advisory Comm, Washington, DC 20585 USA. [Prager, Stewart] APS, Div Plasma Phys, Salt Lake City, UT USA. RP Prager, S (reprint author), Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08544 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA SARA BURGERHARTSTRAAT 25, PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS BN 978-0-08-049271-1 PY 2013 BP 149 EP 164 PG 16 WC Nuclear Science & Technology SC Nuclear Science & Technology GA BEI83 UT WOS:000316751600015 ER PT B AU Prager, S AF Prager, Stewart BA McCracken, G Stott, P BF McCracken, G Stott, P TI Fusion Power Plants SO FUSION: THE ENERGY OF THE UNIVERSE, 2ND EDITION LA English DT Article; Book Chapter C1 [Prager, Stewart] Univ Wisconsin, Madison, WI 53706 USA. [Prager, Stewart] US DOE, Fus Energy Sci Advisory Comm, Washington, DC 20585 USA. [Prager, Stewart] APS, Div Plasma Phys, Salt Lake City, UT USA. RP Prager, S (reprint author), Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08544 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA SARA BURGERHARTSTRAAT 25, PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS BN 978-0-08-049271-1 PY 2013 BP 165 EP 187 PG 23 WC Nuclear Science & Technology SC Nuclear Science & Technology GA BEI83 UT WOS:000316751600016 ER PT B AU Prager, S AF Prager, Stewart BA McCracken, G Stott, P BF McCracken, G Stott, P TI Why We Will Need Fusion Energy SO FUSION: THE ENERGY OF THE UNIVERSE, 2ND EDITION LA English DT Article; Book Chapter C1 [Prager, Stewart] Univ Wisconsin, Madison, WI 53706 USA. [Prager, Stewart] US DOE, Fus Energy Sci Advisory Comm, Washington, DC 20585 USA. [Prager, Stewart] APS, Div Plasma Phys, Salt Lake City, UT USA. RP Prager, S (reprint author), Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08544 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA SARA BURGERHARTSTRAAT 25, PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS BN 978-0-08-049271-1 PY 2013 BP 189 EP 202 PG 14 WC Nuclear Science & Technology SC Nuclear Science & Technology GA BEI83 UT WOS:000316751600017 ER PT J AU Revil, A Skold, M Wu, SSHY Wu, YX Watson, DB Karaoulis, M AF Revil, Andre Skold, Magnus Hubbard, Susan S. Wu, Yuxin Watson, David B. Karaoulis, Marios TI Petrophysical properties of saprolites from the Oak Ridge Integrated Field Research Challenge site, Tennessee SO GEOPHYSICS LA English DT Article ID SPECTRAL INDUCED POLARIZATION; UNSATURATED TRANSPORT PROCESSES; HETEROGENEOUS POROUS-MEDIA; SHALY SANDS; UNCONSOLIDATED SEDIMENTS; COMPLEX CONDUCTIVITY; RESISTIVITY; GROUNDWATER; ADSORPTION; DISPERSION AB At the Oak Ridge Integrated Field Research Challenge site, near Oak Ridge, Tennessee, the shallow saprolitic aquifer is contaminated by nitric acid, uranium, and metals originating from the former S3 settling ponds. To interpret low-frequency geophysical methods used to image contaminant plumes, we have characterized the petrophysical properties of three representative saprolite core samples. Their hydraulic conductivity ranges from 10(-7) to 10(-6) ms(-1) in agreement with field data. Complex conductivity measurements, in the frequency range of 1 mHz to 45 kHz, were performed with NaCl solutions with electrical conductivities in the range 5 x 10(-3) to 2.35 S m(-1), a range representative of field conditions. The electrical conductivity data were well reproduced with a simple linear conductivity model between the saprolite conductivity and the pore water conductivity. The conductivity plots were used to estimate the formation factor (the cementation exponent was about 2.2 +/- 0.3) and the surface conductivity (0.007-0.040 S m(-1)). The magnitude of the surface conductivity depended on the degree of weathering and therefore on the amount of smectite and mixed layer (illite-smectite) clays present in the saprolite. The chargeability of the core samples was in the range of 20 to 800 mV V-1 and is strongly dependent on the salinity. We also performed streaming potential measurements with the same pore fluid composition as that used for the complex conductivity measurements. We found an excess of movable electrical charges on the order of 100 to 500 C m(-3) in agreement with previous investigations connecting the movable excess charge density to permeability. The zeta potential was in the range of -10 to -20 mV independent on the salinity. The electrical measurements were consistent with an average cation exchange capacity in the range of 1.4 to 11 cmol kg(-1) and a specific surface area on the order of 4000 to about 30,000 m(2) kg(-1). C1 [Revil, Andre] Univ Savoie, Le Bourget Du Lac, France. [Revil, Andre; Skold, Magnus; Karaoulis, Marios] Colorado Sch Mines, Dept Geophys, Golden, CO 80401 USA. [Wu, Yuxin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Watson, David B.] Oak Ridge Natl Lab, Oak Ridge, TN USA. RP Revil, A (reprint author), Univ Savoie, Le Bourget Du Lac, France. EM arevil@mines.edu; mskold@mines.edu; sshubbard@lbl.gov; ywu3@lbl.gov; watsondb@ornl.gov; marios.karaoulis@gmail.com RI Hubbard, Susan/E-9508-2010; Watson, David/C-3256-2016; Wu, Yuxin/G-1630-2012 OI Watson, David/0000-0002-4972-4136; Wu, Yuxin/0000-0002-6953-0179 FU U.S. Department of Energy (DOE) [DE-FG02-08ER646559] FX We thank the Environment Remediation Science Program (ERSP), U.S. Department of Energy (DOE), for the funding (award DE-FG02-08ER646559), Richard Wendlandt for XRD analysis, and Manika Prasad for the specific surface area (BET) measurements. We thank Egon Zimmerman for the quality of his impedance meter. We also thank Evert Slob and three anonymous referees for their very constructive reviews. NR 70 TC 19 Z9 19 U1 0 U2 20 PU SOC EXPLORATION GEOPHYSICISTS PI TULSA PA 8801 S YALE ST, TULSA, OK 74137 USA SN 0016-8033 EI 1942-2156 J9 GEOPHYSICS JI Geophysics PD JAN-FEB PY 2013 VL 78 IS 1 BP D21 EP D40 DI 10.1190/GEO2012-0176.1 PG 20 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA 113ND UT WOS:000316673800012 ER PT J AU Tang, JY Riley, WJ AF Tang, J. Y. Riley, W. J. TI A new top boundary condition for modeling surface diffusive exchange of a generic volatile tracer: theoretical analysis and application to soil evaporation SO HYDROLOGY AND EARTH SYSTEM SCIENCES LA English DT Article ID CHEMICAL-TRANSPORT MODEL; BARE-SOIL; POROUS-MEDIA; HYDRAULIC CONDUCTIVITY; BIOGEOCHEMISTRY MODEL; ORGANIC-CHEMICALS; MECHANISTIC MODEL; METHANE EMISSIONS; UNSATURATED SOIL; NUMERICAL-MODEL AB We describe a new top boundary condition (TBC) for representing the air-soil diffusive exchange of a generic volatile tracer. This new TBC (1) accounts for the multi-phase flow of a generic tracer; (2) accounts for effects of soil temperature, pH, solubility, sorption, and desorption processes; (3) enables a smooth transition between wet and dry soil conditions; (4) is compatible with the conductance formulation for modeling air-water volatile tracer exchange; and (5) is applicable to site, regional, and global land models. Based on the new TBC, we developed new formulations for bare-soil resistance and corresponding soil evaporation efficiency. The new soil resistance is predicted as the reciprocal of the harmonic sum of two resistances: (1) gaseous and aqueous molecular diffusion and (2) liquid mass flow resulting from the hydraulic pressure gradient between the soil surface and center of the topsoil control volume. We compared the predicted soil evaporation efficiency with those from several field and laboratory soil evaporation measurements and found good agreement with the typically observed two-stage soil evaporation curves. Comparison with the soil evaporation efficiency equation of Lee and Pielke (1992; hereafter LP92) indicates that their equation can overestimate soil evaporation when the atmospheric resistance is low and underestimate soil evaporation when the soil is dry. Using a synthetic inversion experiment, we demonstrated that using inverted soil resistance data from field measurements to derive empirical soil resistance formulations resulted in large uncertainty because (1) the inverted soil resistance data are always severely impacted by measurement error and (2) the derived empirical equation is very sensitive to the number of data points and the assumed functional form of the resistance. We expect the application of our new TBC in land models will provide a consistent representation for the diffusive tracer exchange at the soil-air interface. C1 [Tang, J. Y.; Riley, W. J.] Lawrence Berkeley Natl Lab LBL, Div Earth Sci, Berkeley, CA USA. RP Tang, JY (reprint author), Lawrence Berkeley Natl Lab LBL, Div Earth Sci, Berkeley, CA USA. EM jinyuntang@lbl.gov RI Tang, Jinyun/M-4922-2013; Riley, William/D-3345-2015 OI Tang, Jinyun/0000-0002-4792-1259; Riley, William/0000-0002-4615-2304 FU Office of Science, Office of Biological and Environmental Research of the US Department of Energy [DE-AC02-05CH11231] FX This research was supported by the Director, Office of Science, Office of Biological and Environmental Research of the US Department of Energy under Contract No. DE-AC02-05CH11231 as part of their Regional and Global Climate Modeling (RGCM) Program. The authors thank Guido Salvucci for his comments on an early version of this manuscript. Discussion with John Selker greatly improved this work. NR 121 TC 11 Z9 11 U1 2 U2 29 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1027-5606 J9 HYDROL EARTH SYST SC JI Hydrol. Earth Syst. Sci. PY 2013 VL 17 IS 2 BP 873 EP 893 DI 10.5194/hess-17-873-2013 PG 21 WC Geosciences, Multidisciplinary; Water Resources SC Geology; Water Resources GA 117NV UT WOS:000316961100016 ER PT J AU Stabley, D Retterer, S Marshall, S Salaita, K AF Stabley, D. Retterer, S. Marshall, S. Salaita, K. TI Manipulating the lateral diffusion of surface-anchored EGF demonstrates that receptor clustering modulates phosphorylation levels SO INTEGRATIVE BIOLOGY LA English DT Article ID EPIDERMAL-GROWTH-FACTOR; PATTERNED LIPID-BILAYERS; CLATHRIN TERMINAL DOMAIN; SIGNAL-TRANSDUCTION; SUPPORTED MEMBRANES; CELL-ACTIVATION; LIVING CELLS; OLIGOMERS; LIGANDS; BINDING AB Upon activation, the epidermal growth factor (EGF) receptor becomes phosphorylated and triggers a vast signaling network that has profound effects on cell growth. The EGF receptor is observed to assemble into clusters after ligand binding and tyrosine kinase autophosphorylation, but the role of these assemblies in the receptor signaling pathway remains unclear. To address this question, we measured the phosphorylation of EGFR when the EGF ligand was anchored onto laterally mobile and immobile surfaces. We found that cells generated clusters of ligand-receptor complex on mobile EGF surfaces, and displayed a lower ratio of phosphorylated EGFR to EGF when compared to immobilized EGF that is unable to cluster. This result was verified by tuning the lateral assembly of ligand-receptor complexes on the surface of living cells using patterned supported lipid bilayers. Nanoscale metal lines fabricated into the supported membrane constrained lipid diffusion and EGF receptor assembly into micron and sub-micron scale corrals. Single cell analysis indicated that clustering impacts EGF receptor activation, and larger clusters (> 1 mm2) of ligand-receptor complex generated lower EGF receptor phosphorylation per ligand than smaller assemblies (o1 mm2) in HCC1143 cells that were engaged to ligand-functionalized surfaces. We investigated the mechanism of EGFR clustering by treating cells with compounds that disrupt the cytoskeleton (Latrunculin B), clathrin-mediated endocytosis (Pitstop2), and inhibit EGFR activation (Gefitinib). These results help elucidate the nature of large-scale EGFR clustering, thus underscoring the general significance of receptor spatial organization in tuning biochemical function. C1 [Stabley, D.; Marshall, S.; Salaita, K.] Emory Univ, Dept Chem, Atlanta, GA 30322 USA. [Retterer, S.] Oak Ridge Natl Lab, Biol & Nanoscale Syst Grp, Oak Ridge, TN USA. RP Stabley, D (reprint author), Emory Univ, Dept Chem, 1515 Pierce Dr, Atlanta, GA 30322 USA. EM k.salaita@emory.edu RI Retterer, Scott/A-5256-2011 OI Retterer, Scott/0000-0001-8534-1979 FU Oak Ridge National Lab Center for Nanophase Materials Sciences [CNMS 2009-269]; National Institutes of Health (NIH) [R01-GM097399-01]; NIH NHLBI Program Excellence in Nanotechnology [HHSN268201000043C]; Emory University Research Committee (URC) [00016401] FX We would like to thank the Oak Ridge National Lab Center for Nanophase Materials Sciences (CNMS 2009-269) for nanofabrication support, and Prof. Jin-Tang Dong at the Winship Cancer Center for the gift of cell lines used herein. K. S. would like to acknowledge support from the National Institutes of Health (NIH) through R01-GM097399-01, seed funding through the NIH NHLBI Program Excellence in Nanotechnology (HHSN268201000043C), and seed funding through the Emory University Research Committee (URC) 00016401. NR 46 TC 13 Z9 13 U1 0 U2 17 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1757-9694 J9 INTEGR BIOL-UK JI Integr. Biol. PY 2013 VL 5 IS 4 BP 659 EP 668 DI 10.1039/c3ib20239a PG 10 WC Cell Biology SC Cell Biology GA 113TX UT WOS:000316692700002 PM 23416883 ER PT J AU Park, CC Georgescu, W Polyzos, A Pham, C Ahmed, KM Zhang, H Costes, SV AF Park, Catherine C. Georgescu, Walter Polyzos, Aris Pham, Christopher Ahmed, Kazi M. Zhang, Hui Costes, Sylvain V. TI Rapid and automated multidimensional fluorescence microscopy profiling of 3D human breast cultures SO INTEGRATIVE BIOLOGY LA English DT Article ID IONIZING-RADIATION; BASEMENT-MEMBRANE; IMAGE-ANALYSIS; 3-DIMENSIONAL CULTURES; CANCER CELLS; IN-VITRO; MORPHOGENESIS; SURVIVAL; GROWTH; MODEL AB Three-dimensional (3D) tissue culture provides a physiologically relevant microenvironment for distinguishing malignant from non-malignant breast cell phenotypes. 3D culture assays can also be used to test novel cancer therapies and predict a differential response to radiation between normal and malignant cells in vivo. However, biological measurements in such complex models are difficult to quantify and current approaches do not allow for in-depth multifaceted assessment of individual colonies or unique sub-populations within the entire culture. This is in part due to the limitations of imaging at a range of depths in 3D culture resulting from optical aberrations and intensity attenuation. Here, we address these limitations by combining sample smearing techniques with high-throughput 2D imaging algorithms to accurately and rapidly quantify imaging features acquired from 3D cultures. Multiple high resolution imaging features especially designed to characterize 3D cultures show that non-malignant human breast cells surviving large doses of ionizing radiation acquire a "swelled acinar'' phenotype with fewer and larger nuclei, loss of cell connectivity and diffused basement membrane. When integrating these imaging features into hierarchical clustering classification, we could also identify subpopulations of phenotypes from individual human tumor colonies treated with ionizing radiation or/and integrin inhibitors. Such tools have therefore the potential to further characterize cell culture populations after cancer treatment and identify novel phenotypes of resistance. C1 [Park, Catherine C.; Georgescu, Walter; Polyzos, Aris; Pham, Christopher; Ahmed, Kazi M.; Zhang, Hui; Costes, Sylvain V.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. [Park, Catherine C.; Ahmed, Kazi M.] Univ Calif San Francisco, Dept Radiat Oncol, San Francisco, CA USA. RP Park, CC (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. EM cpark@radonc.ucsf.edu; svcostes@lbl.gov OI Costes, Sylvain/0000-0002-8542-2389 FU R01 ARRA NIH [CA124891]; Low Dose Scientific Focus Area, United States Department of Energy [DE-AC02-05CH11231]; ICBP program of NCI [U54CA149233] FX This project was mainly supported by a R01 ARRA grant from NIH to CCP [CA124891]. SVC and WG were additionally supported by the Low Dose Scientific Focus Area, United States Department of Energy [DE-AC02-05CH11231] and by the ICBP program of NCI [U54CA149233]. The content is solely the responsibility of the authors and does not necessarily represent the official views of the National Cancer Institute, the National Institutes of Health or the Department of Energy. NR 32 TC 8 Z9 8 U1 0 U2 11 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1757-9694 J9 INTEGR BIOL-UK JI Integr. Biol. PY 2013 VL 5 IS 4 BP 681 EP 691 DI 10.1039/c3ib20275e PG 11 WC Cell Biology SC Cell Biology GA 113TX UT WOS:000316692700005 PM 23407655 ER PT J AU Li, DY Li, N Xia, GF Zheng, Z Wang, JL Xiao, N Zhai, WJ Wu, G AF Li, Deyu Li, Ning Xia, Guofeng Zheng, Zhen Wang, Jialin Xiao, Ning Zhai, Wenjie Wu, Gang TI An in-situ Study of Copper Electropolishing in Phosphoric Acid Solution SO INTERNATIONAL JOURNAL OF ELECTROCHEMICAL SCIENCE LA English DT Article DE copper; electrochemical analysis; electrolytic polishing; ECMP; planarization; surface chemistry ID ELECTROCHEMICAL MECHANICAL PLANARIZATION; ANODIC-DISSOLUTION; CU; H3PO4; FILMS AB In this work, the interface film in the Cu/H3PO4 interface was in-situ studied by tracking the time and potential evolution of the system impedance (R-s) at high-frequency. The fluctuation of R-s upon the applied potentials was confirmed by the R-s-potential plot. A copper oxide film was found formed on the copper surface during the electropolishing process by analyzing the Mott-Schottky curve. Moreover, the copper oxides film exhibited a transition of n-type semiconductor to a p-type one. C1 [Li, Deyu; Li, Ning; Xia, Guofeng; Zheng, Zhen; Wang, Jialin; Xiao, Ning] Harbin Inst Technol, Sch Chem Engn & Technol, Harbin 150001, Peoples R China. [Zhai, Wenjie] Harbin Inst Technol, Sch Mechatron Engn, Harbin 150001, Peoples R China. [Wu, Gang] Los Alamos Natl Lab, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA. RP Li, DY (reprint author), Harbin Inst Technol, Sch Chem Engn & Technol, Harbin 150001, Peoples R China. EM lininghit@263.net RI Wu, Gang/E-8536-2010 OI Wu, Gang/0000-0003-4956-5208 FU National Natural Science Foundation of China [50975058] FX This research was financially supported by National Natural Science Foundation of China (no. 50975058) NR 19 TC 6 Z9 6 U1 10 U2 39 PU ESG PI BELGRADE PA BORIVOJA STEVANOVICA 25-7, BELGRADE, 11000, SERBIA SN 1452-3981 J9 INT J ELECTROCHEM SC JI Int. J. Electrochem. Sci. PD JAN PY 2013 VL 8 IS 1 BP 1041 EP 1046 PG 6 WC Electrochemistry SC Electrochemistry GA 112AE UT WOS:000316562800081 ER PT J AU Sun, Y Tong, C Trainor-Guitton, WJ Lu, C Mansoor, K Carroll, SA AF Sun, Y. Tong, C. Trainor-Guitton, W. J. Lu, C. Mansoor, K. Carroll, S. A. TI Global sampling for integrating physics-specific subsystems and quantifying uncertainties of CO2 geological sequestration SO INTERNATIONAL JOURNAL OF GREENHOUSE GAS CONTROL LA English DT Article DE Uncertainty quantification; CO2 sequestration; Risk assessment; Reactive transport; Global sampling ID DEEP SALINE AQUIFER; SENSITIVITY-ANALYSIS; CARBON-DIOXIDE; SYSTEM MODEL; STORAGE; LEAKAGE; PROBABILITY; MANAGEMENT; CAPACITY; EQUATION AB The risk of CO2 leakage from a deep storage reservoir into a shallow aquifer through a fault is assessed and studied using physics-specific computer models. The hypothetical CO2 geological sequestration system is composed of three subsystems: a deep storage reservoir, a fault in caprock, and a shallow aquifer, which are modeled respectively by considering sub-domain-specific physics. Supercritical CO2 is injected into the reservoir subsystem with uncertain permeabilities of reservoir, caprock, and aquifer, uncertain fault location, and injection rate (as a decision variable). The simulated pressure and CO2/brine saturation are connected to the fault-leakage model as a boundary condition. CO2 and brine fluxes from the fault-leakage model at the fault outlet are then imposed in the aquifer model as a source term. Uncertainties are propagated from the deep reservoir model, to the fault-leakage model, and eventually to the geochemical model in the shallow aquifer, thus contributing to risk profiles. To quantify the uncertainties and assess leakage-relevant risk, we propose a global sampling-based method to allocate sub-dimensions of uncertain parameters to sub-models. The risk profiles are defined and related to CO2 plume development for pH value and total dissolved solids (TDS) below the EPA's Maximum Contaminant Levels (MCL) for drinking water quality. A global sensitivity analysis is conducted to select the most sensitive parameters to the risk profiles. The uncertainty of pH- and TDS-defined aquifer volume, which is impacted by CO2 and brine leakage, mainly results from the uncertainty of fault permeability. Subsequently, high-resolution, reduced-order models of risk profiles are developed as functions of all the decision variables and uncertain parameters in all three subsystems. (C) 2012 Elsevier Ltd. All rights reserved. C1 [Sun, Y.; Tong, C.; Trainor-Guitton, W. J.; Lu, C.; Mansoor, K.; Carroll, S. A.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RP Sun, Y (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94551 USA. EM sun4@llnl.gov RI Sun, Yunwei/C-9751-2010 FU National Risk Assessment Partnership (NRAP); Carbon Capture Simulation Initiative (CCSI) through the National Energy Technology Laboratory; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX The authors wish to thank David Ortiz-Suslow at the University of Miami, Thomas Wolery at Lawrence Livermore National Laboratory, the anonymous reviewer, and the associate editor, Stefan Bachu, for their careful review and constructive comments that led to an improved manuscript. This work was supported in part by the National Risk Assessment Partnership (NRAP) and the Carbon Capture Simulation Initiative (CCSI) through the National Energy Technology Laboratory, and performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under contract DE-AC52-07NA27344. NR 53 TC 12 Z9 13 U1 2 U2 16 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 1750-5836 J9 INT J GREENH GAS CON JI Int. J. Greenh. Gas Control PD JAN PY 2013 VL 12 BP 108 EP 123 DI 10.1016/j.ijggc.2012.10.004 PG 16 WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Energy & Fuels; Engineering, Environmental SC Science & Technology - Other Topics; Energy & Fuels; Engineering GA 109NR UT WOS:000316375800011 ER PT J AU Rinaldi, AP Rutqvist, J AF Rinaldi, Antonio P. Rutqvist, Jonny TI Modeling of deep fracture zone opening and transient ground surface uplift at KB-502 CO2 injection well, In Salah, Algeria SO INTERNATIONAL JOURNAL OF GREENHOUSE GAS CONTROL LA English DT Article ID MULTIPHASE FLUID-FLOW; INDUCED SEISMICITY; CARBON SEQUESTRATION; GEOLOGIC STORAGE; KRECHBA FIELD; RESERVOIR; TECHNOLOGIES; DEFORMATION; AQUIFERS; BEHAVIOR AB The Krechba gas field at In Salah (Algeria), the site of the first industrial scale on-shore CO2 storage demonstration project, is also known for satellite-based ground-deformation monitoring data of remarkable quality. In this work, we focus on the In Salah injection well KB-502, where a double-lobe uplift pattern has been observed in the ground-deformation data. On the basis of previous numerical results, semi-analytical inverse deformation solutions, and seismic analyses, we explain this pattern of uplift as resulting from injection-induced deformation in a deep vertical fracture zone. In this study, we simulate a fracture zone characterized by high permeability and low mechanical stiffness, which activates after a few months of injection, causing irreversible changes in permeability. We study the transient evolution of uplift using the observed injection rate and compare it to the field Interferometric Synthetic Aperture Radar (InSAR) data using the displacement in the satellite line-of-sight. We also carry out a sensitivity study, analyzing the extent of the fracture zone, particularly its height from the reservoir depth. Our analysis supports the notion that the fracture zone is confined within the caprock and does not penetrate into the overlying aquifer. Published by Elsevier Ltd. C1 [Rinaldi, Antonio P.; Rutqvist, Jonny] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Rinaldi, AP (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM aprinaldi@lbl.gov; jrutqvist@lbl.gov RI Rinaldi, Antonio Pio/N-3284-2013; Rutqvist, Jonny/F-4957-2015 OI Rinaldi, Antonio Pio/0000-0001-7052-8618; Rutqvist, Jonny/0000-0002-7949-9785 FU Office of Natural Gas and Petroleum Technology through the National Energy Technology Laboratory; National Energy Technology Laboratory; Sonatrach under the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was jointly supported by the Assistant Secretary for Fossil Energy, Office of Natural Gas and Petroleum Technology, through the National Energy Technology Laboratory, and the In Salah JIP and their partners BP, Statoil, and Sonatrach under the U.S. Department of Energy Contract No. DE-AC02-05CH11231. Technical review comments by Rob Bissell and Lykke Gemmer of the In Salah JIP, and Thomas Daley and Donald Vasco at the Berkeley Lab, as well as editorial review by Dan Hawkes at the Berkeley Lab are all greatly appreciated. We would like to thank two anonymous reviewers for useful comments. NR 46 TC 46 Z9 50 U1 3 U2 33 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 1750-5836 EI 1878-0148 J9 INT J GREENH GAS CON JI Int. J. Greenh. Gas Control PD JAN PY 2013 VL 12 BP 155 EP 167 DI 10.1016/j.ijggc.2012.10.017 PG 13 WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Energy & Fuels; Engineering, Environmental SC Science & Technology - Other Topics; Energy & Fuels; Engineering GA 109NR UT WOS:000316375800015 ER PT J AU Wei, N Li, XC Wang, Y Dahowski, RT Davidson, CL Bromhal, GS AF Wei, Ning Li, Xiaochun Wang, Ying Dahowski, Robert T. Davidson, Casie L. Bromhal, Grant S. TI A preliminary sub-basin scale evaluation framework of site suitability for onshore aquifer-based CO2 storage in China SO INTERNATIONAL JOURNAL OF GREENHOUSE GAS CONTROL LA English DT Article DE Site suitability evaluation; CO2 storage; Multi-criteria analysis; Onshore aquifers ID DEEP SALINE AQUIFERS; SEDIMENTARY BASINS; GEOLOGICAL STORAGE; CARBON-DIOXIDE; CLIMATE-CHANGE; EARLY OPPORTUNITIES; EASTERN CHINA; BOHAI BASIN; COST CURVE; LONG-TERM AB Development of a reliable, broadly applicable framework for the identification and suitability evaluation of potential CO2 storage sites is essential before large-scale deployment of carbon dioxide capture and geological storage (CCS) can commence. In this study, a sub-basin scale evaluation framework was developed to assess the suitability of potential onshore deep saline aquifers for CO2 storage in China. The methodology, developed in consultation with experts from the academia and the petroleum industry in China, is based on a multi-criteria analysis (MCA) framework that considers four objectives: (1) storage optimization, in terms of storage capacity and injectivity; (2) risk minimization and storage security; (3) environmental restrictions regarding surface and subsurface use; and (4) economic considerations. The framework is designed to provide insights into both the suitability of potential aquifer storage sites as well as the priority for early deployment of CCS with existing CO2 sources. Preliminary application of the framework, conducted using GIS-based evaluation tools revealed that 18% of onshore aquifer sites with a combined CO2 storage capacity of 746 gigatons are considered to exhibit very high suitability, and 11% of onshore aquifer sites with a total capacity of 290 gigatons exhibit very high priority opportunities for implementation. These onshore aquifer sites may provide promising opportunities for early large-scale CCS deployment and contribute to CO2 mitigation in China for many decades. (C) 2012 Elsevier Ltd. All rights reserved. C1 [Wei, Ning; Li, Xiaochun; Wang, Ying] Chinese Acad Sci, Inst Rock & Soil Mech, State Key Lab Geomech & Geotech Engn, Wuhan 430071, Peoples R China. [Dahowski, Robert T.; Davidson, Casie L.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Bromhal, Grant S.] Natl Energy Technol Lab, Morgantown, WV USA. RP Li, XC (reprint author), Chinese Acad Sci, Inst Rock & Soil Mech, State Key Lab Geomech & Geotech Engn, Wuhan 430071, Peoples R China. EM nwei@whrsm.ac.cn; Xcli@whrsm.ac.cn FU Energy Foundation-Beijing Office [G-0810-10457]; Projects of International Cooperation from Ministry of Science and Technology of China; Joint Research on Low Emission Technologies for Integrated Gasification Combined Cycle [2010DFB70560] FX The authors would like to acknowledge the financial support provided by the Energy Foundation-Beijing Office (Grant number: G-0810-10457) and the support by Projects of International Cooperation from Ministry of Science and Technology of China, Joint Research on Low Emission Technologies for Integrated Gasification Combined Cycle (Grant number: 2010DFB70560). The authors would also like to acknowledge all the experts from the Ministry of Land and Resources of the People's Republic of China, petroleum companies, universities, the Chinese Academy of Sciences, and other institutions, for their valued input and suggestions, as well as the reviewers for their thoughtful and helpful comments. NR 62 TC 17 Z9 19 U1 2 U2 25 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 1750-5836 J9 INT J GREENH GAS CON JI Int. J. Greenh. Gas Control PD JAN PY 2013 VL 12 BP 231 EP 246 DI 10.1016/j.ijggc.2012.10.012 PG 16 WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Energy & Fuels; Engineering, Environmental SC Science & Technology - Other Topics; Energy & Fuels; Engineering GA 109NR UT WOS:000316375800022 ER PT J AU Zhang, KL Li, XHS Duan, YH King, DL Singh, P Li, LY AF Zhang, Keling Li, Xiaohong S. Duan, Yuhua King, David L. Singh, Prabhakar Li, Liyu TI Roles of double salt formation and NaNO3 in Na2CO3-promoted MgO absorbent for intermediate temperature CO2 removal SO INTERNATIONAL JOURNAL OF GREENHOUSE GAS CONTROL LA English DT Article DE CO2 absorption and desorption; Na2CO3 promoted MgO; Na2Mg(CO3)(2) double salt; Warm temperature CO2 capture; Pre-combustion CO2 capture; NaNO3 facilitated CO2 capture ID CAPTURE; SORBENTS; NITRITE; NITRATE AB Absorption and desorption of carbon dioxide on Na2CO3-promoted MgO have been studied at temperatures compatible with warm gas cleanup (300-470 degrees C) from a pre-combustion syngas. The absorbents are synthesized through the formation and activation of the precipitate resulting from the addition of sodium carbonate to an aqueous solution of magnesium nitrate. The absorbent, which comprises MgO, Na2CO3 and residual NaNO3 after activation, forms the double salt Na2Mg(CO3)(2) on exposure to CO2. The thermodynamic properties of the double salt, obtained through computational calculation, predict that the preferred temperature range for absorption of CO2 with the double salt is significantly higher compared with MgO. Faster CO2 uptake can be achieved as a result of this higher temperature absorption window. Absorption tests indicate that the double salt absorbent as prepared has a capacity toward CO2 of 15 wt.% (3.4 mmol CO2/g absorbent) and can be easily regenerated through both pressure swing and temperature swing absorption in multiple-cycle tests. Thermodynamic calculations also predict an important effect of CO2 partial pressure on the absorption capacity in the warm temperature range. The impurity phase, NaNO3, is identified as a key component in facilitating CO2 absorption by these materials. The reason for reported difficulties in reproducing the performance of these materials can be traced to specific details of the synthesis method, which are reviewed in some detail. (C) 2012 Elsevier Ltd. All rights reserved. C1 [Zhang, Keling; Singh, Prabhakar] Univ Connecticut, Ctr Clean Energy Engn, Storrs, CT 06269 USA. [Zhang, Keling; Singh, Prabhakar] Univ Connecticut, Dept Chem Mat & Biomol Engn, Storrs, CT 06269 USA. [Li, Xiaohong S.; King, David L.; Li, Liyu] Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99354 USA. [Duan, Yuhua] US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. RP King, DL (reprint author), Pacific NW Natl Lab, Inst Integrated Catalysis, P 0 Box 999, Richland, WA 99354 USA. EM David.King@pnnl.gov RI Singh, Prabhakar/M-3186-2013; Duan, Yuhua/D-6072-2011 OI Duan, Yuhua/0000-0001-7447-0142 FU US DOE Office of Fossil Energy (NETL); US DOE (EERE) Office of Biomass; State of Wyoming; PNNL internal investment (LDRD-ECI); DOE's Office of Biological and Environmental Research (BER) FX Financial support from the US DOE Office of Fossil Energy (NETL), the US DOE (EERE) Office of Biomass, the State of Wyoming, and PNNL internal investment (LDRD-ECI) is gratefully acknowledged. Some work was carried out at the Environmental and Molecular Science Laboratory, a national scientific user facility sponsored by the DOE's Office of Biological and Environmental Research (BER). NR 18 TC 32 Z9 35 U1 5 U2 45 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 1750-5836 J9 INT J GREENH GAS CON JI Int. J. Greenh. Gas Control PD JAN PY 2013 VL 12 BP 351 EP 358 DI 10.1016/j.ijggc.2012.11.013 PG 8 WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Energy & Fuels; Engineering, Environmental SC Science & Technology - Other Topics; Energy & Fuels; Engineering GA 109NR UT WOS:000316375800033 ER PT J AU Sullivan, EJ Chu, SP Stauffer, PH Middleton, RS Pawar, RJ AF Sullivan, Enid J. Chu, Shaoping Stauffer, Philip H. Middleton, Richard S. Pawar, Rajesh J. TI A method and cost model for treatment of water extracted during geologic CO2 storage SO INTERNATIONAL JOURNAL OF GREENHOUSE GAS CONTROL LA English DT Article DE Reverse osmosis; Nanofiltration; Multiple-effect distillation; Multistage flash distillation; Thermal distillation; Brine concentrate disposal ID CARBON-DIOXIDE; SYSTEM MODEL; SEQUESTRATION; DESALINATION; CAPTURE; CHALLENGES; MSF AB Extraction of water as a part of CO2 storage may be desirable for risk management and process optimization. Treatment and repurposing of this water creates a useful resource and reduces the volumes that must otherwise be disposed. To better understand the tradeoff of costs versus processes and risks, we use a systems approach to evaluate treatment costs that are reasonable for the chemical and physical qualities (salinity, temperature, pH and turbidity) of water that could be extracted from target geologic formations. We evaluate primary and secondary pretreatments, membrane desalination processes (reverse osmosis and nanofiltration), thermal processes (multiple effect distillation and multi-stage flash distillation), and several concentrate (brine) disposal methods. The results indicate that for waters extracted from storage sites, salinities and temperatures may often be higher than for municipal treatment scenarios. Thus, thermal treatment methods are more cost-feasible than membrane methods in many cases, although pressure recovery methods for reverse osmosis can mitigate this. Treatment costs including concentrate disposal fall within a range of US$0.50-2.50/ton CO2 injected, although some costs can be much higher (up to US$30/ton CO2 under certain concentrate disposal cost ranges). A sensitivity analysis shows that temperature is the most important in determining costs followed by selection of concentrate disposal method. (C) 2012 Elsevier Ltd. All rights reserved. C1 [Sullivan, Enid J.] Los Alamos Natl Lab, Chem Diagnost & Engn Grp, Los Alamos, NM 87544 USA. [Chu, Shaoping; Stauffer, Philip H.; Middleton, Richard S.; Pawar, Rajesh J.] Los Alamos Natl Lab, Computat Earth Sci Grp, Los Alamos, NM USA. RP Sullivan, EJ (reprint author), Los Alamos Natl Lab, C CDE Grp, MS J964, Los Alamos, NM 87545 USA. EM ejs@lanl.gov; spchu@lanl.gov; stauffer@lanl.gov; rsm@lanl.gov; pawar@lanl.gov OI Stauffer, Philip/0000-0002-6976-221X FU US DOE's Office of Fossil Energy through National Energy Technology Laboratory's Carbon Sequestration Program FX This work was funded by the US DOE's Office of Fossil Energy through the National Energy Technology Laboratory's Carbon Sequestration Program. NR 49 TC 11 Z9 11 U1 0 U2 10 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 1750-5836 J9 INT J GREENH GAS CON JI Int. J. Greenh. Gas Control PD JAN PY 2013 VL 12 BP 372 EP 381 DI 10.1016/j.ijggc.2012.11.007 PG 10 WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Energy & Fuels; Engineering, Environmental SC Science & Technology - Other Topics; Energy & Fuels; Engineering GA 109NR UT WOS:000316375800035 ER PT J AU Kazakov, AE Rodionov, DA Price, MN Arkin, AP Dubchak, I Novichkov, PS AF Kazakov, Alexey E. Rodionov, Dmitry A. Price, Morgan N. Arkin, Adam P. Dubchak, Inna Novichkov, Pavel S. TI Transcription Factor Family-Based Reconstruction of Singleton Regulons and Study of the Crp/Fnr, ArsR, and GntR Families in Desulfovibrionales Genomes SO JOURNAL OF BACTERIOLOGY LA English DT Article ID MYCOBACTERIUM-SMEGMATIS; STAPHYLOCOCCUS-AUREUS; REGULATORY NETWORKS; METABOLISM; SEQUENCE; IDENTIFICATION; PROKARYOTES; INFERENCE; PATTERNS; BACTERIA AB Accurate detection of transcriptional regulatory elements is essential for high-quality genome annotation, metabolic reconstruction, and modeling of regulatory networks. We developed a computational approach for reconstruction of regulons operated by transcription factors (TFs) from large protein families and applied this novel approach to three TF families in 10 Desulfovibrionales genomes. Phylogenetic analyses of 125 regulators from the ArsR, Crp/Fnr, and GntR families revealed that 65% of these regulators (termed reference TFs) are well conserved in Desulfovibrionales, while the remaining 35% of regulators (termed singleton TFs) are species specific and show a mosaic distribution. For regulon reconstruction in the group of singleton TFs, the standard orthology-based approach was inefficient, and thus, we developed a novel approach based on the simultaneous study of all homologous TFs from the same family in a group of genomes. As a result, we identified binding for 21 singleton TFs and for all reference TFs in all three analyzed families. Within each TF family we observed structural similarities between DNA-binding motifs of different reference and singleton TFs. The collection of reconstructed regulons is available at the RegPrecise database (http://regprecise.lbl.gov/RegPrecise/Desulfovibrionales.jsp). C1 [Kazakov, Alexey E.; Price, Morgan N.; Arkin, Adam P.; Dubchak, Inna; Novichkov, Pavel S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Kazakov, Alexey E.; Rodionov, Dmitry A.] Russian Acad Sci, AA Kharkevich Inst Informat Transmiss Problems, Moscow, Russia. [Rodionov, Dmitry A.] Sanford Burnham Med Res Inst, La Jolla, CA USA. RP Kazakov, AE (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM aekazakov@lbl.gov; psnovichkov@lbl.gov RI Arkin, Adam/A-6751-2008; OI Arkin, Adam/0000-0002-4999-2931; Rodionov, Dmitry/0000-0002-0939-390X; Price, Morgan/0000-0002-4251-0362 FU Office of Science, Office of Biological and Environmental Research, of the U.S. Department of Energy [DE-AC02-05CH11231]; Lawrence Berkeley National Laboratory (ENIGMA SFA); Sanford-Burnham Medical Research Institute [DE-SC0004999]; Lawrence Berkeley National Laboratory; Russian Foundation for Basic Research [10-04-01768] FX This research was supported by the Office of Science, Office of Biological and Environmental Research, of the U.S. Department of Energy under contracts DE-AC02-05CH11231 with Lawrence Berkeley National Laboratory (ENIGMA SFA), and DE-SC0004999 with Sanford-Burnham Medical Research Institute and Lawrence Berkeley National Laboratory. D.A.R. was also supported by the Russian Foundation for Basic Research (10-04-01768). NR 30 TC 11 Z9 11 U1 1 U2 10 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 0021-9193 J9 J BACTERIOL JI J. Bacteriol. PD JAN PY 2013 VL 195 IS 1 BP 29 EP 38 DI 10.1128/JB.01977-12 PG 10 WC Microbiology SC Microbiology GA 117NA UT WOS:000316959000006 PM 23086211 ER PT J AU Lennen, RM Politz, MG Kruziki, MA Pfleger, BF AF Lennen, Rebecca M. Politz, Mark G. Kruziki, Max A. Pfleger, Brian F. TI Identification of Transport Proteins Involved in Free Fatty Acid Efflux in Escherichia coli SO JOURNAL OF BACTERIOLOGY LA English DT Article ID ORGANIC-SOLVENT TOLERANCE; P-BAD PROMOTER; OUTER-MEMBRANE; MULTIDRUG-RESISTANCE; CELL-ENVELOPE; GENES; PUMP; EXPRESSION; TOLC; OVERPRODUCTION AB Escherichia coli has been used as a platform host for studying the production of free fatty acids (FFA) and other energy-dense compounds useful in biofuel applications. Most of the FFA produced by E. coli are found extracellularly. This finding suggests that a mechanism for transport across the cell envelope exists, yet knowledge of proteins that may be responsible for export remains incomplete. Production of FFA has been shown to cause cell lysis, induce stress responses, and impair basic physiological processes. These phenotypes could potentially be diminished if efflux rates were increased. Here, a total of 15 genes and operons were deleted and screened for their impact on cell viability and titer in FFA-producing E. coli. Deletions of acrAB and rob and, to a lower degree of statistical confidence, emrAB, mdtEF, and mdtABCD reduced multiple measures of viability, while deletion of tolC nearly abolished FFA production. An acrAB emrAB deletion strain exhibited greatly reduced FFA titers approaching the tolC deletion phenotype. Expression of efflux pumps on multicopy plasmids did not improve endogenous FFA production in an acrAB(+) strain, but plasmid-based expression of acrAB, mdtEF, and an mdtEF-tolC artificial operon improved the MIC of exogenously added decanoate for an acrAB mutant strain. The findings suggest that AcrAB-TolC is responsible for most of the FFA efflux in E. coli, with residual activity provided by other resistance-nodulation-cell division superfamily-type efflux pumps, including EmrAB-TolC and MdtEF-TolC. While the expression of these proteins on multicopy plasmids did not improve production over the basal level, their identification enables future engineering efforts. C1 [Lennen, Rebecca M.; Politz, Mark G.; Kruziki, Max A.; Pfleger, Brian F.] Univ Wisconsin Madison, Dept Chem & Biol Engn, Madison, WI 53715 USA. [Lennen, Rebecca M.; Pfleger, Brian F.] Univ Wisconsin Madison, US DOE, Great Lakes Bioenergy Res Ctr, Madison, WI USA. RP Pfleger, BF (reprint author), Univ Wisconsin Madison, Dept Chem & Biol Engn, Madison, WI 53715 USA. EM pfleger@engr.wisc.edu FU DOE Great Lakes Bioenergy Research Center (DOE BER Office of Sciences) [DE-FC02-07ER64494]; Chemistry-Biology Interface Training Program (NIH); Department of Chemical and Biological Engineering Dahlke-Hougen Fellowship; Holstrom Environmental Research Scholarship (University of Wisconsin-Madison); Biotechnology Training Program (NIH) FX This work was funded by the DOE Great Lakes Bioenergy Research Center (DOE BER Office of Sciences DE-FC02-07ER64494). R.M.L. was supported as a trainee in the Chemistry-Biology Interface Training Program (NIH) and by the Department of Chemical and Biological Engineering Dahlke-Hougen Fellowship. M.A.K. was the recipient of a Holstrom Environmental Research Scholarship (University of Wisconsin-Madison). M.G.P. was supported as a trainee in the Biotechnology Training Program (NIH). NR 67 TC 29 Z9 30 U1 2 U2 50 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 0021-9193 J9 J BACTERIOL JI J. Bacteriol. PD JAN PY 2013 VL 195 IS 1 BP 135 EP 144 DI 10.1128/JB.01477-12 PG 10 WC Microbiology SC Microbiology GA 117NA UT WOS:000316959000017 PM 23104810 ER PT J AU Motl, NE Mann, AKP Skrabalak, SE AF Motl, Nathan E. Mann, Amanda K. P. Skrabalak, Sara E. TI Aerosol-assisted synthesis and assembly of nanoscale building blocks SO JOURNAL OF MATERIALS CHEMISTRY A LA English DT Article ID ULTRASONIC SPRAY-PYROLYSIS; SILICA PARTICLES; NANOPARTICLE FORMATION; MICROFLUIDIC SYNTHESIS; CONTINUOUS-FLOW; FLAME-SYNTHESIS; GRAPHENE OXIDE; DROPLETS; ROUTE; NANOCRYSTALS AB Aerosol methods, including spray drying and spray pyrolysis, represent industrial scale routes to materials on account of their continuous nature. Recently, these methods have been used to prepare size-, shape- and architecturally controlled nanostructures for a range of inorganic materials. In this Feature Article, a brief overview of traditional aerosol methods is provided. Then, the new chemical methods that have been integrated into aerosol techniques to achieve high quality nanomaterials are highlighted. Given that the properties of nanomaterials are dependent on their structural features, these synthetic advances help to address the critical need for new nanomanufacturing routes to materials. C1 [Motl, Nathan E.; Skrabalak, Sara E.] Indiana Univ, Dept Chem, Bloomington, IN 47405 USA. [Mann, Amanda K. P.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN USA. RP Motl, NE (reprint author), Indiana Univ, Dept Chem, Bloomington, IN 47405 USA. EM nmotl@indiana.edu; mannak@ornl.gov; sskrabal@indiana.edu FU Indiana University; ACS-PRF [48790-DNI10]; NSF [DMR-0955028] FX We acknowledge financial support from Indiana University, ACS-PRF 48790-DNI10, and NSF CAREER DMR-0955028. NR 87 TC 13 Z9 13 U1 5 U2 61 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2050-7488 EI 2050-7496 J9 J MATER CHEM A JI J. Mater. Chem. A PY 2013 VL 1 IS 17 BP 5193 EP 5202 DI 10.1039/c3ta01703f PG 10 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Energy & Fuels; Materials Science GA 117QK UT WOS:000316968000001 ER PT J AU Chen, HP Chen, JH Yin, W Yu, X Shao, M Xiao, K Hong, KL Pickel, DL Kochemba, WM Kilbey, SM Dadmun, M AF Chen, Huipeng Chen, Jihua Yin, Wen Yu, Xiang Shao, Ming Xiao, Kai Hong, Kunlun Pickel, Deanna L. Kochemba, W. Michael Kilbey, S. Michael, II Dadmun, Mark TI Correlation of polymeric compatibilizer structure to its impact on the morphology and function of P3HT:PCBM bulk heterojunctions SO JOURNAL OF MATERIALS CHEMISTRY A LA English DT Article ID ANGLE NEUTRON-SCATTERING; PLASTIC SOLAR-CELLS; REGIOREGULAR POLY(3-HEXYLTHIOPHENE); INTERPENETRATING NETWORK; ORGANIC PHOTOVOLTAICS; CONJUGATED POLYMER; DIBLOCK COPOLYMER; MOLECULAR-WEIGHT; EFFICIENCY; PERFORMANCE AB The impact of various polymeric compatibilizers, including end-functionalized P3HTs and diblock copolymers containing P3HT, on the structure and function of poly(3-hexylthiophene) (P3HT):[6,6]phenyl-C61-butyric acid methyl ester (PCBM) bulk heterojunctions is presented. Careful analyses of small angle neutron scattering curves provide a measure of the miscibility of PCBM in P3HT, the average PCBM domain size, and the interfacial area between PCBM and the P3HT-rich phase in the uncompatibilized and compatibilized systems. Differential scanning calorimetry (DSC) also provides information regarding the changes in the crystallinity of P3HT due to the presence of the compatibilizer. Results show that most compatibilizers cause the domain sizes to decrease and the P3HT crystallinity to increase; however, some cause an increase in domain size, suggesting that they are not effective interfacial modifiers. The correlation of morphology with photovoltaic activity shows that the decreased domain size, increased crystallinity and increased interfacial area do not always result in improved power conversion efficiency (PCE). It appears that the introduction of an insulating molecule at the PCBM: P3HT interface as a compatibilizer results in a decrease in PCE. Thus, the presence of the compatibilizer at this interface dominates the photovoltaic activity, rather than the morphological control. C1 [Chen, Huipeng; Yin, Wen; Kochemba, W. Michael; Kilbey, S. Michael, II; Dadmun, Mark] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Chen, Jihua; Shao, Ming; Xiao, Kai; Hong, Kunlun; Pickel, Deanna L.; Kilbey, S. Michael, II] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Yu, Xiang; Dadmun, Mark] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. RP Chen, HP (reprint author), Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. EM dad@utk.edu RI Chen, Jihua/F-1417-2011; Chen, Huipeng/G-4019-2012; Hong, Kunlun/E-9787-2015 OI Chen, Jihua/0000-0001-6879-5936; Hong, Kunlun/0000-0002-2852-5111 FU Sustainable Energy Education Research Center; Joint Institute for Neutron Sciences at the University of Tennessee; National Science Foundation [DMR-1005987]; Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; TN-SCORE; NSF-EPSCOR [EPS-1004083] FX The authors wish to acknowledge the Sustainable Energy Education Research Center and the Joint Institute for Neutron Sciences at the University of Tennessee, as well as the National Science Foundation (DMR-1005987) for support of this project. MDD also acknowledges the support of the Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. A portion of this research was conducted at the Center for Nanophase Materials Sciences and High Flux Isotope Reactor, which are sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. In addition, SMK and WMK acknowledge support from TN-SCORE, a multi-disciplinary research program sponsored by NSF-EPSCOR (EPS-1004083). NR 55 TC 17 Z9 17 U1 5 U2 65 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2050-7488 J9 J MATER CHEM A JI J. Mater. Chem. A PY 2013 VL 1 IS 17 BP 5309 EP 5319 DI 10.1039/c3ta10386b PG 11 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Energy & Fuels; Materials Science GA 117QK UT WOS:000316968000018 ER PT J AU Akilavasan, J Wijeratne, K Moutinho, H Al-Jassim, M Alamoud, ARM Rajapakse, RMG Bandara, J AF Akilavasan, Jeganathan Wijeratne, Kosala Moutinho, Hellio Al-Jassim, Mowafak Alamoud, A. R. M. Rajapakse, R. M. G. Bandara, Jayasundera TI Hydrothermally synthesized titania nanotubes as a promising electron transport medium in dye sensitized solar cells exhibiting a record efficiency of 7.6% for 1-D based devices SO JOURNAL OF MATERIALS CHEMISTRY A LA English DT Article ID TIO2 NANOTUBES; ENHANCED EFFICIENCY; LIGHT-SCATTERING; ARRAYS; FABRICATION; FILM; NANOSTRUCTURES; NANOPARTICLES; PERFORMANCE; CONVERSION AB Hydrothermally synthesized TiO2 nanotubes (TNTs) with a diameter of approximately 10 nm and a length of 250 nm are successfully employed in dye-sensitized solar cells (DSSCs) based on N719 dye and iodide/triiodide electrolyte and exhibiting an efficiency of 7.6% at 1 sun illumination. Randomly oriented TiO2 nanotubes are deposited on FTO glass by the electrophoretic deposition method, and the thickness of the TNT layer and hence the solar cell performance have been shown to depend on the deposition time and the nanotube concentration in the electrolyte solution. The highest efficiency is obtained for the solar cell fabricated with the 6-minute electrophoretically deposited TiO2 film having a film thickness of similar to 6 mm. These pristine TNT photoelectrodes exhibit a short-circuit current density (J(sc)), an open-circuit voltage (V-oc), a fill factor (FF) and an efficiency (eta) of 2.4 mA cm(-2), 899 mV, 78% and 1.7%, respectively. TiCl4 treatment of pristine TNT photoelectrodes enhances the J(sc), V-oc, FF and eta to 13.2 mA cm(-2), 819 mV, 70.4% and 7.6%, respectively. The TiCl4 treatment is found to be vital for the enhancement of the solar cell performance of hydrothermally synthesised TiO2 nanotube based devices. Enhancement of electron lifetime is noted after treatment of bare TiO2 nanotubes with 0.5 M TiCl4 solution. The electron transport resistance, electron lifetime and charge recombination properties of bare and TiCl4 treated TiO2 nanotubes are investigated by electrochemical impedance measurements. The increased performance of the DSSC fabricated with TiCl4 treated TNTs is due to several factors favouring the enhancement of efficiency. These include the dye loading amount, the decrease in electron transport resistance, the increase in density of states and enhancement of light scattering. C1 [Akilavasan, Jeganathan; Wijeratne, Kosala; Bandara, Jayasundera] Inst Fundamental Studies, Kandy, Sri Lanka. [Moutinho, Hellio; Al-Jassim, Mowafak] NREL, Golden, CO 80401 USA. [Alamoud, A. R. M.] King Saud Univ, Dept Elect Engn, Riyadh, Ksa, Saudi Arabia. [Rajapakse, R. M. G.] Univ Peradeniya, Dept Chem, Peradeniya, Sri Lanka. RP Akilavasan, J (reprint author), Inst Fundamental Studies, Hantana Rd,CP20000, Kandy, Sri Lanka. EM jayasundera@yahoo.com FU NRC, Sri Lanka [NRC 07-46]; AvH Foundation, Germany FX Financial support (NRC 07-46) from NRC, Sri Lanka, is highly appreciated. A research grant from AvH Foundation, Germany, to purchase the electrochemical workstation is highly appreciated. JB appreciates the Visiting Professor Program of King Saud University, Riyadh, KSA. NR 39 TC 21 Z9 21 U1 4 U2 33 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2050-7488 J9 J MATER CHEM A JI J. Mater. Chem. A PY 2013 VL 1 IS 17 BP 5377 EP 5385 DI 10.1039/c3ta01576a PG 9 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Energy & Fuels; Materials Science GA 117QK UT WOS:000316968000027 ER PT J AU Chang, C Sustarich, J Bharadwaj, R Chandrasekaran, A Adams, PD Singh, AK AF Chang, Chieh Sustarich, Jess Bharadwaj, Rajiv Chandrasekaran, Aarthi Adams, Paul D. Singh, Anup K. TI Droplet-based microfluidic platform for heterogeneous enzymatic assays SO LAB ON A CHIP LA English DT Article ID IONIC LIQUIDS; CELLULASE; OPTIMIZATION; REGENERATION; PRETREATMENT; SWITCHGRASS; CONFINEMENT; DISSOLUTION; HYDROLYSIS; BACTERIA AB Heterogeneous enzymatic reactions are used in many industrial processes including pulp and paper, food, and biofuel production. Industrially-relevant optimization of the enzymes used in these processes requires assaying them with insoluble substrates. However, platforms for high throughput heterogeneous assays do not exist thereby severely increasing the cost and time of enzyme optimization, or leading to the use of assays with soluble substrates for convenient, but non-ideal, optimization. We present an innovative approach to perform heterogeneous reactions in a high throughput fashion using droplet microfluidics. Droplets provide a facile platform for heterogeneous reactions as internal recirculation allows rapid mixing of insoluble substrates with soluble enzymes. Moreover, it is easy to generate hundreds or thousands of picoliter droplets in a small footprint chip allowing many parallel reactions. We validate our approach by screening combinations of cellulases with real-world insoluble substrates, and demonstrate that the chip-based screening is in excellent agreement with the conventional screening methods, while offering advantages of throughput, speed and lower reagent consumption. We believe that our approach, while demonstrated for a biofuel application, provides a generic platform for high throughput monitoring of heterogeneous reactions. C1 [Chang, Chieh; Sustarich, Jess; Bharadwaj, Rajiv; Chandrasekaran, Aarthi; Adams, Paul D.; Singh, Anup K.] Joint BioEnergy Inst, Technol Div, Emeryville, CA 94608 USA. [Chang, Chieh; Sustarich, Jess; Bharadwaj, Rajiv; Chandrasekaran, Aarthi; Singh, Anup K.] Sandia Natl Labs, Biotechnol & Bioengn Dept, Livermore, CA 94551 USA. RP Singh, AK (reprint author), Joint BioEnergy Inst, Technol Div, 5885 Hollis St, Emeryville, CA 94608 USA. EM aksingh@sandia.gov RI Adams, Paul/A-1977-2013 OI Adams, Paul/0000-0001-9333-8219 FU US Department of Energy, Office of Science, Office of Biological and Environmental Research [DE-AC02-05CH11231]; United States Department of Energy's Nuclear Security Administration [DE-AC04-94AL85000] FX This work was part of the DOE Joint BioEnergy Institute, supported by the US Department of Energy, Office of Science, Office of Biological and Environmental Research, through contract DE-AC02-05CH11231 between Lawrence Berkeley National Laboratory and the US Department of Energy. Sandia is a multi-program laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy's Nuclear Security Administration under contract DE-AC04-94AL85000. NR 38 TC 14 Z9 14 U1 8 U2 71 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1473-0197 J9 LAB CHIP JI Lab Chip PY 2013 VL 13 IS 9 BP 1817 EP 1822 DI 10.1039/c3lc41418c PG 6 WC Biochemical Research Methods; Chemistry, Multidisciplinary; Nanoscience & Nanotechnology SC Biochemistry & Molecular Biology; Chemistry; Science & Technology - Other Topics GA 117OL UT WOS:000316962700020 PM 23507976 ER PT J AU Wang, P Tartakovsky, DM Jarman, KD Tartakovsky, AM AF Wang, P. Tartakovsky, D. M. Jarman, K. D., Jr. Tartakovsky, A. M. TI CDF SOLUTIONS OF BUCKLEY-LEVERETT EQUATION WITH UNCERTAIN PARAMETERS SO MULTISCALE MODELING & SIMULATION LA English DT Article DE uncertainty quantification; Buckley-Leverett equation; multiphase flow; probability density function; cumulative density function; oil recovery ID HETEROGENEOUS POROUS-MEDIA; PROBABILISTIC COLLOCATION; STOCHASTIC-ANALYSIS; IMMISCIBLE FLOW; SPARSE GRIDS; DISPLACEMENT; TRANSPORT; 2-PHASE AB The Buckley-Leverett (nonlinear advection) equation is often used to describe two-phase flow in porous media. We develop a new probabilistic method to quantify parametric uncertainty in the Buckley- Leverett model. Our approach is based on the concept of a fine-grained cumulative density function (CDF) and provides a full statistical description of the system states. Hence, it enables one to obtain not only average system response but also the probability of rare events, which is critical for risk assessment. We obtain a closed-form, semianalytical solution for the CDF of the state variable (fluid saturation) and test it against the results from Monte Carlo simulations. C1 [Wang, P.; Jarman, K. D., Jr.; Tartakovsky, A. M.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Tartakovsky, D. M.] Univ Calif San Diego, Dept Mech & Aerosp Engn, La Jolla, CA 92093 USA. RP Wang, P (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM Peng.Wang@pnnl.gov; dmt@ucsd.edu; kj@pnnl.gov; alexandre.tartakovsky@pnnl.gov RI Tartakovsky, Daniel/E-7694-2013; Jarman, Kenneth/B-6157-2011 OI Jarman, Kenneth/0000-0002-4396-9212 FU Office of Advanced Scientific Computing Research; U.S. Department of Energy; U.S. Department of Energy [DE-AC05-76RL01830] FX Received by the editors February 10, 2012; accepted for publication (in revised form) September 20, 2012; published electronically January 15, 2013. This work was supported by the Office of Advanced Scientific Computing Research funded by the U.S. Department of Energy. Pacific Northwest National Laboratory is operated by Battelle for the U.S. Department of Energy under contract DE-AC05-76RL01830. The U.S. Government retains a nonexclusive, royalty-free license to publish or reproduce the published form of this contribution, or allow others to do so, for U.S. Government purposes. Copyright is owned by SIAM to the extent not limited by these rights. NR 34 TC 6 Z9 6 U1 0 U2 5 PU SIAM PUBLICATIONS PI PHILADELPHIA PA 3600 UNIV CITY SCIENCE CENTER, PHILADELPHIA, PA 19104-2688 USA SN 1540-3459 J9 MULTISCALE MODEL SIM JI Multiscale Model. Simul. PY 2013 VL 11 IS 1 BP 118 EP 133 DI 10.1137/120865574 PG 16 WC Mathematics, Interdisciplinary Applications; Physics, Mathematical SC Mathematics; Physics GA 116CY UT WOS:000316861400005 ER PT J AU Liu, KH Hong, XP Wu, MH Xiao, FJ Wang, WL Bai, XD Ager, JW Aloni, S Zettl, A Wang, EG Wang, F AF Liu, Kaihui Hong, Xiaoping Wu, Muhong Xiao, Fajun Wang, Wenlong Bai, Xuedong Ager, Joel W. Aloni, Shaul Zettl, Alex Wang, Enge Wang, Feng TI Quantum-coupled radial-breathing oscillations in double-walled carbon nanotubes SO NATURE COMMUNICATIONS LA English DT Article ID MODE; SPECTROSCOPY; SCATTERING; CHAINS; LAYERS AB Van der Waals-coupled materials, ranging from multilayers of graphene and MoS2 to superlattices of nanoparticles, exhibit rich emerging behaviour owing to quantum coupling between individual nanoscale constituents. Double-walled carbon nanotubes provide a model system for studying such quantum coupling mediated by van derWaals interactions, because each constituent single-walled nanotube can have distinctly different physical structures and electronic properties. Here we systematically investigate quantum-coupled radial-breathing mode oscillations in chirality-defined double-walled nanotubes by combining simultaneous structural, electronic and vibrational characterizations on the same individual nanotubes. We show that these radial-breathing oscillations are collective modes characterized by concerted inner-and outer-wall motions, and determine quantitatively the tube-dependent van der Waals potential governing their vibration frequencies. We also observe strong quantum interference between Raman scattering from the inner-and outer-wall excitation pathways, the relative phase of which reveals chirality-dependent excited-state potential energy surface displacement in different nanotubes. C1 [Liu, Kaihui; Hong, Xiaoping; Xiao, Fajun; Zettl, Alex; Wang, Feng] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Liu, Kaihui; Wu, Muhong; Wang, Wenlong; Bai, Xuedong] Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China. [Ager, Joel W.; Zettl, Alex; Wang, Feng] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Aloni, Shaul] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Wang, Enge] Peking Univ, Sch Phys, Int Ctr Quantum Mat, Beijing 100871, Peoples R China. RP Wang, F (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM fengwang76@berkeley.edu RI Hong, Xiaoping/G-8673-2013; Liu, Kaihui/A-9938-2014; Foundry, Molecular/G-9968-2014; Zettl, Alex/O-4925-2016; wang, Feng/I-5727-2015; OI Hong, Xiaoping/0000-0002-5864-4533; Zettl, Alex/0000-0001-6330-136X; Ager, Joel/0000-0001-9334-9751 FU NSF [0846648, DMR10-1006184]; NSF Centre for Integrated Nanomechanical Systems [EEC-0832819]; DOE [DE-AC02-05CH11231]; DOE Molecular Foundry [DE-AC02-05CH11231]; MOST [2012CB933003]; CAS [KJCX2-YW-M13, KJCX2-YW-W35]; NSF of China [11027402, 91021007, 10974238, 20973195] FX This study was supported by NSF CAREER grant (No. 0846648), NSF Centre for Integrated Nanomechanical Systems (No. EEC-0832819), NSF Grant No. DMR10-1006184, DOE Contract No. DE-AC02-05CH11231 and DOE Molecular Foundry (No. DE-AC02-05CH11231); and by the MOST (Grant No. 2012CB933003), CAS (Grant Nos. KJCX2-YW-M13 and KJCX2-YW-W35) and NSF (Grant Nos. 11027402, 91021007, 10974238 and 20973195) of China. NR 33 TC 15 Z9 15 U1 4 U2 134 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD JAN PY 2013 VL 4 AR 1375 DI 10.1038/ncomms2367 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 112SV UT WOS:000316614600045 PM 23340415 ER PT J AU Miller, TA Wittenberg, JS Wen, H Connor, S Cui, Y Lindenberg, AM AF Miller, T. A. Wittenberg, J. S. Wen, H. Connor, S. Cui, Y. Lindenberg, A. M. TI The mechanism of ultrafast structural switching in superionic copper (I) sulphide nanocrystals SO NATURE COMMUNICATIONS LA English DT Article ID NA BETA-ALUMINA; LOW CHALCOCITE; CRYSTAL-STRUCTURES; QUANTUM DOTS; PHASE; DYNAMICS; CU2S; TRANSITION; TRANSFORMATIONS; TEMPERATURE AB Superionic materials are multi-component solids with simultaneous characteristics of both a solid and a liquid. Above a critical temperature associated with a structural phase transition, they exhibit liquid-like ionic conductivities and dynamic disorder within a rigid crystalline structure. Broad applications as electrochemical storage materials and resistive switching devices follow from this abrupt change in ionic mobility, but the microscopic pathways and speed limits associated with this switching process are largely unknown. Here we use ultrafast X-ray spectroscopy and scattering techniques to obtain an atomic-level, real-time view of the transition state in copper sulphide nanocrystals. We observe the transformation to occur on a twenty picosecond timescale and show that this is determined by the ionic hopping time. C1 [Miller, T. A.; Wittenberg, J. S.; Connor, S.; Cui, Y.; Lindenberg, A. M.] Stanford Univ, Dept Mat Sci & Engn, Stanford, CA 94305 USA. [Wen, H.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Lindenberg, A. M.] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. RP Lindenberg, AM (reprint author), Stanford Univ, Dept Mat Sci & Engn, Stanford, CA 94305 USA. EM aaronl@stanford.edu RI WEN, HAIDAN/B-5258-2009; Miller, Timothy/C-9128-2011 OI Miller, Timothy/0000-0002-5585-7736 FU U. S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division; Office of Science, Office of Basic Energy Sciences of the U. S. Department of Energy [DE-AC02-05CH11231]; U. S. DOE [DE-AC02-06CH11357] FX Research was supported by the U. S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division, and performed in part at the Advanced Light Source, the Advanced Photon Source and the Stanford Synchrotron Radiation Lightsource, DOE-BES user facilities. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences of the U. S. Department of Energy under contract number DE-AC02-05CH11231. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U. S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U. S. DOE under contract number DE-AC02-06CH11357. Portions of this research were carried out at the Stanford Synchrotron Radiation Lightsource, a Directorate of SLAC National Accelerator Laboratory and an Office of Science User Facility operated for the U. S. Department of Energy Office of Science by Stanford University. We are grateful for the experimental assistance of T. E. Glover and M. Hertlein at Lawrence Berkeley National Laboratory, as well as N. Huse for useful discussion. NR 47 TC 28 Z9 28 U1 5 U2 127 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD JAN PY 2013 VL 4 AR 1369 DI 10.1038/ncomms2385 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 112SV UT WOS:000316614600039 PM 23340409 ER PT J AU Ryan, PJ Kim, JW Birol, T Thompson, P Lee, JH Ke, X Normile, PS Karapetrova, E Schiffer, P Brown, SD Fennie, CJ Schlom, DG AF Ryan, P. J. Kim, J. -W. Birol, T. Thompson, P. Lee, J. -H. Ke, X. Normile, P. S. Karapetrova, E. Schiffer, P. Brown, S. D. Fennie, C. J. Schlom, D. G. TI Reversible control of magnetic interactions by electric field in a single-phase material SO NATURE COMMUNICATIONS LA English DT Article ID FERROELECTRICITY; MULTIFERROICS; POLARIZATION; PEROVSKITES; DOMAINS AB Intrinsic magnetoelectric coupling describes the interaction between magnetic and electric polarization through an inherent microscopic mechanism in a single-phase material. This phenomenon has the potential to control the magnetic state of a material with an electric field, an enticing prospect for device engineering. Here, we demonstrate 'giant' magnetoelectric cross-field control in a tetravalent titanate film. In bulk form, EuTiO3, is anti-ferromagnetic. However, both anti and ferromagnetic interactions coexist between different nearest europium neighbours. In thin epitaxial films, strain was used to alter the relative strength of the magnetic exchange constants. We not only show that moderate biaxial compression precipitates local magnetic competition, but also demonstrate that the application of an electric field at this strain condition switches the magnetic ground state. Using first-principles density functional theory, we resolve the underlying microscopic mechanism resulting in G-type magnetic order and illustrate how it is responsible for the 'giant' magnetoelectric effect. C1 [Ryan, P. J.; Kim, J. -W.; Lee, J. -H.; Karapetrova, E.] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. [Birol, T.; Fennie, C. J.] Cornell Univ, Sch Appl Engn Phys, Ithaca, NY 14853 USA. [Thompson, P.; Brown, S. D.] Univ Liverpool, Dept Phys, Liverpool L69 3BX, Merseyside, England. [Thompson, P.; Brown, S. D.] European Synchrotron Radiat Facil, XMaS, F-38043 Grenoble, France. [Ke, X.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Normile, P. S.] Univ Castilla La Mancha, IRICA, E-13071 Ciudad Real, Spain. [Normile, P. S.] Univ Castilla La Mancha, Dept Fis Aplicada, E-13071 Ciudad Real, Spain. [Schiffer, P.] Penn State Univ, Dept Phys, University Pk, PA 16802 USA. [Schiffer, P.] Penn State Univ, Mat Res Inst, University Pk, PA 16802 USA. [Schlom, D. G.] Cornell Univ, Dept Mat Sci & Engn, Ithaca, NY 14853 USA. RP Ryan, PJ (reprint author), Argonne Natl Lab, Xray Sci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM pryan@aps.anl.gov RI Birol, Turan/D-1948-2012; Schlom, Darrell/J-2412-2013; Normile, Peter/I-2320-2015; OI Birol, Turan/0000-0001-5174-3320; Schlom, Darrell/0000-0003-2493-6113; Normile, Peter/0000-0002-8851-9899; Schiffer, Peter/0000-0002-6430-6549 FU US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; EPSRC; PSU MRSEC [DMR-0820404]; DOE-BES [DE-SCOO02334] FX Work at Argonne and use of beamline 6-ID-B at the Advanced Photon Source at Argonne was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences under Contract No. DE-AC02-06CH11357. The EPSRC-funded XMaS beamline at the ESRF is directed by M.J. Cooper, C. A. Lucas and T. P. A. Hase. P. S., X. K., J.-H.L. and D. G. S were funded through PSU MRSEC, Grant DMR-0820404. T. B. and C.J.F. were supported by the DOE-BES under Grant No. DE-SCOO02334. P.J.R. is grateful for fruitful discussions with Jonathon Lang, Steve May, John W. Freeland, Andreas Kreyssig and Yusuke Wakabayashi. Additional thanks to Michael Wieczorek, Chian Liu, and Michael McDowell, David Gagliano for sample processing and sample environment engineering, respectively. We are grateful to O. Bikondoa, D. Wermeille and L. Bouchenoire for their invaluable assistance, and to S. Beaufoy and J. Kervin for additional XMaS support. NR 42 TC 31 Z9 31 U1 4 U2 132 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD JAN PY 2013 VL 4 AR 1334 DI 10.1038/ncomms2329 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 112SV UT WOS:000316614600004 PM 23299884 ER PT J AU Si, WD Han, SJ Shi, XY Ehrlich, SN Jaroszynski, J Goyal, A Li, Q AF Si, Weidong Han, Su Jung Shi, Xiaoya Ehrlich, Steven N. Jaroszynski, J. Goyal, Amit Li, Qiang TI High current superconductivity in FeSe0.5Te0.5-coated conductors at 30 tesla SO NATURE COMMUNICATIONS LA English DT Article ID NB3SN AB Although high-temperature superconductor cuprates have been discovered for more than 25 years, superconductors for high-field application are still based on low-temperature superconductors, such as Nb3Sn. The high anisotropies, brittle textures and high manufacturing costs limit the applicability of the cuprates. Here we demonstrate that the iron superconductors, without most of the drawbacks of the cuprates, have a superior high-field performance over low-temperature superconductors at 4.2 K. With a CeO2 buffer, critical current densities >10(6) A cm(-2) were observed in iron-chalcogenide FeSe0.5Te0.5 films grown on single-crystalline and coated conductor substrates. These films are capable of carrying critical current densities exceeding 10(5) A cm(-2) under 30 tesla magnetic fields, which are much higher than those of low-temperature superconductors. High critical current densities, low magnetic field anisotropies and relatively strong grain coupling make iron-chalcogenide-coated conductors particularly attractive for high-field applications at liquid helium temperatures. C1 [Si, Weidong; Han, Su Jung; Shi, Xiaoya; Li, Qiang] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Ehrlich, Steven N.] Brookhaven Natl Lab, Natl Synchrotron Light Source, Upton, NY 11973 USA. [Jaroszynski, J.] Florida State Univ, Natl High Magnet Field Natl Lab, Tallahassee, FL 32310 USA. [Goyal, Amit] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Si, WD (reprint author), Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. EM wds@bnl.gov; qiangli@bnl.gov FU US Department of Energy, Office of Basic Energy Science, Materials Sciences and Engineering Division [DE-AC0298CH10886]; US Department of Energy, Office of Electricity; US Department of Energy; National Science Foundation [DMR-0654118]; State of Florida FX This work was supported by the US Department of Energy, Office of Basic Energy Science, Materials Sciences and Engineering Division, under contract no. DE-AC0298CH10886. RABiTS is a registered trademark of Oak Ridge National Laboratory (ORNL). The RABiTS templates were fabricated at ORNL under funding from the US Department of Energy, Office of Electricity. A portion of this work was performed at the National Synchrotron Light Source (NSLS) and the National High Magnetic Field Laboratory (NHMFL). NSLS is funded by the US Department of Energy. NHMFL is supported by National Science Foundation Cooperative Agreement No. DMR-0654118, the State of Florida and the US Department of Energy. NR 27 TC 63 Z9 65 U1 9 U2 84 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD JAN PY 2013 VL 4 AR 1347 DI 10.1038/ncomms2337 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 112SV UT WOS:000316614600017 PM 23299897 ER PT J AU Yu, KY Bufford, D Sun, C Liu, Y Wang, H Kirk, MA Li, M Zhang, X AF Yu, K. Y. Bufford, D. Sun, C. Liu, Y. Wang, H. Kirk, M. A. Li, M. Zhang, X. TI Removal of stacking-fault tetrahedra by twin boundaries in nanotwinned metals SO NATURE COMMUNICATIONS LA English DT Article ID HELIUM ION-IRRADIATION; DEFECT ACCUMULATION; RADIATION-DAMAGE; STAINLESS-STEEL; VOID FORMATION; GRAIN-SIZE; COPPER; DISLOCATIONS; MICROSTRUCTURE; MULTILAYERS AB Stacking-fault tetrahedra are detrimental defects in neutron-or proton-irradiated structural metals with face-centered cubic structures. Their removal is very challenging and typically requires annealing at very high temperatures, incorporation of interstitials or interaction with mobile dislocations. Here we present an alternative solution to remove stacking-fault tetrahedra discovered during room temperature, in situ Kr ion irradiation of epitaxial nanotwinned Ag with an average twin spacing of similar to 8 nm. A large number of stacking-fault tetrahedra were removed during their interactions with abundant coherent twin boundaries. Consequently the density of stacking-fault tetrahedra in irradiated nanotwinned Ag was much lower than that in its bulk counterpart. Two fundamental interaction mechanisms were identified, and compared with predictions by molecular dynamics simulations. In situ studies also revealed a new phenomenon: radiation-induced frequent migration of coherent and incoherent twin boundaries. Potential migration mechanisms are discussed. C1 [Yu, K. Y.; Bufford, D.; Sun, C.; Liu, Y.; Zhang, X.] Texas A&M Univ, Dept Mech Engn, Mat Sci & Engn Program, College Stn, TX 77843 USA. [Wang, H.] Texas A&M Univ, Dept Elect & Comp Engn, College Stn, TX 77843 USA. [Kirk, M. A.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Li, M.] Argonne Natl Lab, Nucl Engn Div, Argonne, IL 60439 USA. RP Zhang, X (reprint author), Texas A&M Univ, Dept Mech Engn, Mat Sci & Engn Program, College Stn, TX 77843 USA. EM zhangx@tamu.edu RI Sun, Cheng/G-8953-2013; Yu, Kaiyuan /B-8398-2014; Liu, Yue/H-4071-2014; Wang, Haiyan/P-3550-2014 OI Sun, Cheng/0000-0002-1368-243X; Yu, Kaiyuan /0000-0002-5442-2992; Liu, Yue/0000-0001-8518-5734; Wang, Haiyan/0000-0002-7397-1209 FU US Army Research Office-Materials Science Division [W911NF-09-1-0223]; DOE-NEUP [DE-AC07-05ID14517-00088120]; NSF-DMR metallic materials and nanostructures programme [0644835]; DOE-BES FX We acknowledge financial support by US Army Research Office-Materials Science Division, under contract no. W911NF-09-1-0223 and partial support by DOE-NEUP under contract no. DE-AC07-05ID14517-00088120, and NSF-DMR metallic materials and nanostructures programme, under grant no. 0644835. We also thank Edward A. Ryan and Peter M. Baldo at Argonne National Laboratory for their help during in situ experiments. The IVEM facility at Argonne National Laboratory is supported by DOE-BES. NR 38 TC 51 Z9 52 U1 12 U2 134 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD JAN PY 2013 VL 4 AR 1377 DI 10.1038/ncomms2382 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 112SV UT WOS:000316614600047 PM 23340417 ER PT S AU Yablonovitch, E Miller, OD Kurtz, SR AF Yablonovitch, Eli Miller, Owen D. Kurtz, Sarah R. BE Linke, H Borgstrom, M Pullerits, T Samuelson, L Sundstrom, V Inganas, O TI A Great Solar Cell also Needs to be a Great LED: External Fluorescence Leads to New Efficiency Record SO NOBEL SYMPOSIUM 153: NANOSCALE ENERGY CONVERTERS SE AIP Conference Proceedings LA English DT Proceedings Paper CT Nobel Symposium 153 on Nanoscale Energy Converters CY AUG 12-16, 2012 CL SWEDEN SP Nobel Fdn AB Counter-intuitively, efficient external fluorescence is a necessity for achieving the highest possible solar cell efficiency. Why would a solar cell, which is intended to absorb light, benefit from emitting light? Although it is tempting to equate light emission with loss, paradoxically, light emission actually improves the open-circuit voltage, and the efficiency. C1 [Yablonovitch, Eli; Miller, Owen D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Kurtz, Sarah R.] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Yablonovitch, E (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RI Miller, Owen/A-6354-2014 OI Miller, Owen/0000-0003-2745-2392 NR 4 TC 2 Z9 2 U1 3 U2 24 PU AMER INST PHYSICS PI MELVILLE PA 2 HUNTINGTON QUADRANGLE, STE 1NO1, MELVILLE, NY 11747-4501 USA SN 0094-243X BN 978-0-7354-1142-5 J9 AIP CONF PROC PY 2013 VL 1519 BP 9 EP 11 DI 10.1063/1.4794698 PG 3 WC Nanoscience & Nanotechnology; Physics, Applied SC Science & Technology - Other Topics; Physics GA BEJ42 UT WOS:000316902100002 ER PT S AU Olson, JM AF Olson, J. M. BE Linke, H Borgstrom, M Pullerits, T Samuelson, L Sundstrom, V Inganas, O TI Multijunction solar cells for concentrator applications SO NOBEL SYMPOSIUM 153: NANOSCALE ENERGY CONVERTERS SE AIP Conference Proceedings LA English DT Proceedings Paper CT Nobel Symposium 153 on Nanoscale Energy Converters CY AUG 12-16, 2012 CL SWEDEN SP Nobel Fdn ID GAAS; GAP C1 Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Olson, JM (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. NR 17 TC 0 Z9 0 U1 0 U2 3 PU AMER INST PHYSICS PI MELVILLE PA 2 HUNTINGTON QUADRANGLE, STE 1NO1, MELVILLE, NY 11747-4501 USA SN 0094-243X BN 978-0-7354-1142-5 J9 AIP CONF PROC PY 2013 VL 1519 BP 22 EP 25 DI 10.1063/1.4794701 PG 4 WC Nanoscience & Nanotechnology; Physics, Applied SC Science & Technology - Other Topics; Physics GA BEJ42 UT WOS:000316902100005 ER PT S AU Tsao, JY AF Tsao, J. Y. BE Linke, H Borgstrom, M Pullerits, T Samuelson, L Sundstrom, V Inganas, O TI Ultra-Efficient Solid-State Lighting: Likely Characteristics, Economic Benefits, Technological Approaches SO NOBEL SYMPOSIUM 153: NANOSCALE ENERGY CONVERTERS SE AIP Conference Proceedings LA English DT Proceedings Paper CT Nobel Symposium 153 on Nanoscale Energy Converters CY AUG 12-16, 2012 CL SWEDEN SP Nobel Fdn AB Technologies for artificial lighting have made tremendous progress over the centuries. At this point in time, there is virtually no question that solid-state lighting (SSL) will eventually displace its predecessor technologies(1). A remaining question, however, is what the final efficiency of SSL will be. In this talk, we give a perspective on the future of SSL, with a focus on ultra-high(2)(>70%) efficiencies. We ask, and sketch answers to, three questions. First, what are some of the likely characteristics of ultra-efficient SSL? Second, what are some of the economic benefits of ultra-efficient SSL? And, third, what are some of the challenges associated with various possible technological approaches to ultra-efficient SSL? C1 Sandia Natl Labs, Phys Chem & Nano Sci Ctr, Albuquerque, NM 87122 USA. RP Tsao, JY (reprint author), Sandia Natl Labs, Phys Chem & Nano Sci Ctr, POB 5800, Albuquerque, NM 87122 USA. NR 11 TC 0 Z9 0 U1 0 U2 4 PU AMER INST PHYSICS PI MELVILLE PA 2 HUNTINGTON QUADRANGLE, STE 1NO1, MELVILLE, NY 11747-4501 USA SN 0094-243X BN 978-0-7354-1142-5 J9 AIP CONF PROC PY 2013 VL 1519 BP 32 EP 35 DI 10.1063/1.4794703 PG 4 WC Nanoscience & Nanotechnology; Physics, Applied SC Science & Technology - Other Topics; Physics GA BEJ42 UT WOS:000316902100007 ER PT J AU Tao, LY Davis, R Heyer, N Yang, QL Qiu, W Zhu, LL Li, N Zhang, H Zeng, L Zhao, YM AF Tao, Liyuan Davis, Robert Heyer, Nicholas Yang, Qiuling Qiu, Wei Zhu, Liangliang Li, Nan Zhang, Hua Zeng, Lin Zhao, Yiming TI Effect of cigarette smoking on noise-induced hearing loss in workers exposed to occupational noise in China SO NOISE & HEALTH LA English DT Article DE Cigarette smoking; hearing loss; occupational noise exposure study ID RISK-FACTORS; IMPAIRMENT; AGE; POPULATION; VISCOSITY; BLOOD AB Excessive exposure to high noise level environments has the potential to cause noise-induced hearing loss (NIHL), and cigarette smoking has also been shown to have a potential adverse effect on hearing. The aim of this study was to determine whether smoking interacts with noise in the development of hearing loss, and if so, the extent of the contribution from smoking on NIHL. A cross-sectional study was designed to assess the effect of smoking on NIHL in 517 male workers (non-smokers: N = 199; smokers: N = 318) exposed to a high-level industrial noise environment in China. Shift-long temporal waveforms of the noise that workers were exposed to for evaluation of noise exposures, and audiometric threshold measures were obtained on all selected subjects. The subjects used hearing protection devices only within the last 1-2 years. The results suggest that smoking has an adverse effect on NIHL in workers exposed to high level industrial noise, i.e., the median high frequency hearing thresholds were significantly greater in smokers than non-smokers exposed to noise for more than 10 years. This effect was observed at 4.0 and 6.0 kHz. Smoking did not have an adverse effect on NIHL in workers exposed to noise less than 10 years. Multivariate regression analysis revealed that the odds ratio (OR) for high frequency hearing loss (i.e., hearing threshold greater than 40 dB at 4.0 kHz) were 1.94 for smokers in comparison to non-smokers. The results suggest that: (1) smokers have a higher risk of developing high frequency hearing loss than non-smokers with a similar occupational noise exposure, and (2) the interaction between cigarette smoking and high-level noise exposure may be additive. There is a need to develop and analyze a larger database of workers with well-documented exposures and smoking histories for better understanding of the effect of smoking on NIHL incurred from high-level industrial noise exposures. A better understanding of the role of smoking may lead to its incorporation into hearing risk assessment for noise exposure. C1 [Tao, Liyuan; Li, Nan; Zhang, Hua; Zeng, Lin; Zhao, Yiming] Peking Univ, Hosp 3, Res Ctr Clin Epidemiol, Beijing 100191, Peoples R China. [Tao, Liyuan; Zhao, Yiming] Peking Univ, Hosp 3, Res Ctr Occupat Med, Beijing 100191, Peoples R China. [Davis, Robert; Qiu, Wei] SUNY Coll Plattsburgh, Auditory Res Lab, Plattsburgh, NY 12901 USA. [Heyer, Nicholas] Battelle Ctr Publ Hlth Res, Seattle, WA USA. [Heyer, Nicholas] Battelle Ctr Evaluat, Seattle, WA USA. [Yang, Qiuling; Zhu, Liangliang] Dongfeng Inst Occupat Dis Prevent, Shi Yan 442001, Peoples R China. RP Zhao, YM (reprint author), Peking Univ, Hosp 3, Res Ctr Occupat Med, Res Ctr Clin Epidemiol, Beijing 100191, Peoples R China. EM yimingzhao115@163.com FU National Institute for Occupational Safety and Health [1-R01-OH-002317] FX Source of Support: Grant No. 1-R01-OH-002317, National Institute for Occupational Safety and Health, Conflict of Interest: None declared. NR 39 TC 10 Z9 13 U1 0 U2 16 PU MEDKNOW PUBLICATIONS & MEDIA PVT LTD PI MUMBAI PA B-9, KANARA BUSINESS CENTRE, OFF LINK RD, GHAKTOPAR-E, MUMBAI, 400075, INDIA SN 1463-1741 J9 NOISE HEALTH JI Noise Health PD JAN-FEB PY 2013 VL 15 IS 62 BP 67 EP 72 DI 10.4103/1463-1741.107159 PG 6 WC Audiology & Speech-Language Pathology; Public, Environmental & Occupational Health SC Audiology & Speech-Language Pathology; Public, Environmental & Occupational Health GA 114QB UT WOS:000316756000009 PM 23412581 ER PT J AU Lin, X Wang, ZT Lyubinetsky, I Kay, BD Dohnalek, Z AF Lin, Xiao Wang, Zhi-Tao Lyubinetsky, Igor Kay, Bruce D. Dohnalek, Zdenek TI Interaction of CO2 with oxygen adatoms on rutile TiO2(110) SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID PHOTOCATALYTIC REDUCTION; CARBON-DIOXIDE; O-2 DISSOCIATION; SURFACE SCIENCE; OXIDE SURFACES; ADSORPTION; H2O; WATER; DYNAMICS; SITES AB The interactions of CO2 with oxygen adatoms (O-a's) on rutile TiO2(110) surfaces have been studied using scanning tunneling microscopy. At 50 K CO2 is found to adsorb preferentially on five-coordinated Ti sites (Ti-5c's) next to O-a's rather than on oxygen vacancies (V-O's) (the most stable adsorption sites on reduced TiO2(110)). Temperature dependent studies show that after annealing to 100-160 K, V-O's become preferentially populated indicating the presence of a kinetic barrier for CO2 adsorption onto the V-O's. The difference between the CO2 binding energy on V-O's and Ti-5c sites next to the O-a's is found to be only 0.009-0.025 eV. The barrier for CO2 diffusion away from O-a's is estimated to be similar to 0.17 eV. Crescent-like features of the images of CO2 adsorbed on Ti-5c's next to O-a's are interpreted as a time average of terminally bound CO2 molecules switching between the configurations that are tilted towards O-a and/or towards one of the two neighbouring bridging oxygen (O-b) rows. In the presence of V-O defects, the Ti-5c bound CO2 is found to tilt preferentially away from the V-O containing Ob row. If another CO2 is present on the neighbouring Ti-5c row, both CO2 molecules tilt towards the common O-b row that separates them. C1 [Lin, Xiao; Kay, Bruce D.; Dohnalek, Zdenek] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. [Lin, Xiao; Kay, Bruce D.; Dohnalek, Zdenek] Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99352 USA. [Wang, Zhi-Tao; Lyubinetsky, Igor] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. RP Dohnalek, Z (reprint author), Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, POB 999, Richland, WA 99352 USA. EM Zdenek.Dohnalek@pnnl.gov RI Lin, Xiao/B-5055-2009 FU Laboratory Directed Research and Development (LDRD) Program at Pacific Northwest National Laboratory (PNNL); Chemical Imaging LDRD; US Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences Biosciences; Department of Energy's Office of Biological and Environmental Research FX X.L. is grateful for the support of the Linus Pauling Distinguished Postdoctoral Fellowship Program funded by Laboratory Directed Research and Development (LDRD) Program at Pacific Northwest National Laboratory (PNNL). Z.W. and I.L. were supported by the Chemical Imaging LDRD, others by the US Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences & Biosciences. PNNL is a multiprogram national laboratory operated for DOE by Battelle. A portion of the research was performed using EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. NR 44 TC 8 Z9 8 U1 5 U2 86 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PY 2013 VL 15 IS 17 BP 6190 EP 6195 DI 10.1039/c3cp44040k PG 6 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 118GN UT WOS:000317012800007 PM 23364757 ER PT J AU Liu, B Greeley, J AF Liu, Bin Greeley, Jeffrey TI A density functional theory analysis of trends in glycerol decomposition on close-packed transition metal surfaces SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID BIOMASS-DERIVED HYDROCARBONS; INITIO MOLECULAR-DYNAMICS; TOTAL-ENERGY CALCULATIONS; FINDING SADDLE-POINTS; MODIFIED NI CATALYSTS; AUGMENTED-WAVE METHOD; WATER-GAS SHIFT; METHANOL DECOMPOSITION; C-C; OXYGENATED HYDROCARBONS AB We describe an accelerated density functional theory (DFT)-based computational strategy to determine trends in the decomposition of glycerol via elementary dehydrogenation, C-C, and C-O bond scission reactions on close-packed transition metal surfaces. Beginning with periodic DFT calculations on Pt(111), the thermochemistry of glycerol dehydrogenation on Pd(111), Rh(111), Cu(111) and Ni(111) is determined using a parameter-free, bond order-based scaling relationship. By combining the results with Bronsted-Evans-Polanyi (BEP) relationships to estimate elementary reaction barriers, free energy diagrams are developed on the respective metal surfaces, and trends concerning the relative selectivity and activity for C-C and C-O bond scission in glycerol on the various metals are obtained. The results are consistent with available theoretical and experimental literature and demonstrate that scaling relationships are capable of providing powerful insights into the catalytic chemistry of complex biomolecules. C1 [Liu, Bin] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Liu, Bin] Kansas State Univ, Dept Chem Engn, Manhattan, KS 66506 USA. [Greeley, Jeffrey] Purdue Univ, Sch Chem Engn, W Lafayette, IN 47907 USA. RP Greeley, J (reprint author), Purdue Univ, Sch Chem Engn, W Lafayette, IN 47907 USA. EM jgreeley@purdue.edu RI Liu, Bin/C-1475-2012 FU Institute for Atom-efficient Chemical Transformations (IACT), an Energy Frontier Research Center; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences; Office of Science of the US Department of Energy [DE-AC02-06CH11357]; EMSL, a national scientific user facility located at Pacific Northwest National Laboratory; NERSC, the user facility located at Lawrence Berkeley National Laboratory; Argonne Laboratory Computing Resource Center (LCRC) FX This work is supported as part of the Institute for Atom-efficient Chemical Transformations (IACT), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. Use of the Center for Nanoscale Materials (CNM) is supported by the Office of Science of the US Department of Energy under contract No. DE-AC02-06CH11357. The authors acknowledge grants of computer time from EMSL, a national scientific user facility located at Pacific Northwest National Laboratory, NERSC, the user facility located at Lawrence Berkeley National Laboratory, and the Argonne Laboratory Computing Resource Center (LCRC). NR 62 TC 23 Z9 23 U1 5 U2 94 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PY 2013 VL 15 IS 17 BP 6475 EP 6485 DI 10.1039/c3cp44088e PG 11 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 118GN UT WOS:000317012800040 PM 23529559 ER PT J AU Gao, ZM Daw, CS Wagner, RM Edwards, KD Smith, DE AF Gao, Zhiming Daw, C. Stuart Wagner, Robert M. Edwards, K. Dean Smith, David E. TI Simulating the impact of premixed charge compression ignition on light-duty diesel fuel economy and emissions of particulates and NOx SO PROCEEDINGS OF THE INSTITUTION OF MECHANICAL ENGINEERS PART D-JOURNAL OF AUTOMOBILE ENGINEERING LA English DT Article DE Diesel oxidation catalyst; lean nitrogen oxide trap; diesel particulate filter; diesel emissions; premixed charge compression ignition; dual-mode engine; transient driving cycle ID ENGINE; COMBUSTION; HCCI; TEMPERATURE; REDUCTION; MODEL AB We report results from urban drive cycle simulations of a light-duty conventional vehicle and a similar hybrid electric vehicle, both of which are equipped with diesel engines capable of operating in either conventional diesel combustion mode or in premixed charge compression ignition mode. Both simulated vehicles include lean exhaust after-treatment trains for controlling hydrocarbon, carbon monoxide, nitrogen oxide, and particulate matter emissions. Our results indicate that, in the simulated conventional vehicle, premixed charge compression ignition can significantly reduce fuel consumption and emissions by reducing the need for lean nitrogen oxide traps and diesel particulate filter regeneration. However, the opportunity for utilizing premixed charge compression ignition in the simulated hybrid electric vehicle is limited because the engine typically experiences higher loads and multiple stop-start transients that are outside the allowable premixed charge compression ignition operating range. This suggests that developing ways of extending the premixed charge compression ignition operating range combined with improved control strategies for engine and emissions control management will be especially important for realizing the potential benefits of premixed charge compression ignition in hybrid electric vehicles. C1 [Gao, Zhiming; Daw, C. Stuart; Wagner, Robert M.; Edwards, K. Dean; Smith, David E.] Oak Ridge Natl Lab, Fuels Engines & Emiss Res Ctr, Knoxville, TN 37932 USA. RP Gao, ZM (reprint author), Oak Ridge Natl Lab, Fuels Engines & Emiss Res Ctr, 2360 Cherahala Blvd, Knoxville, TN 37932 USA. EM gaoz@ornl.gov OI Gao, Zhiming/0000-0002-7139-7995 FU United States Government [DE-AC05-00OR22725]; United States Department of Energy FX This submission was sponsored by a contractor of the United States Government under contract DE-AC05-00OR22725 with the United States Department of Energy. The United States Government retains, and the publisher, by accepting this submission for publication, acknowledges that the United States Government retains, a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this submission, or allow others to do so, for United States Government purposes. NR 54 TC 5 Z9 5 U1 1 U2 14 PU SAGE PUBLICATIONS LTD PI LONDON PA 1 OLIVERS YARD, 55 CITY ROAD, LONDON EC1Y 1SP, ENGLAND SN 0954-4070 J9 P I MECH ENG D-J AUT JI Proc. Inst. Mech. Eng. Part D-J. Automob. Eng. PY 2013 VL 227 IS 1 SI SI BP 31 EP 51 DI 10.1177/0954407012459137 PG 21 WC Engineering, Mechanical; Transportation Science & Technology SC Engineering; Transportation GA 114SM UT WOS:000316762700004 ER PT J AU Wallner, T Matthias, NS Scarcelli, R Kwon, JC AF Wallner, Thomas Matthias, Nicholas S. Scarcelli, Riccardo Kwon, Jason C. TI Evaluation of the efficiency and the drive cycle emissions for a hydrogen direct-injection engine SO PROCEEDINGS OF THE INSTITUTION OF MECHANICAL ENGINEERS PART D-JOURNAL OF AUTOMOBILE ENGINEERING LA English DT Article DE Hydrogen internal-combustion engine; hydrogen direct-injection engine; FreedomCAR; light-duty targets; brake thermal efficiency; engine maps; alternative fuel; gaseous fuel; vehicle simulation; fuel economy; nitrogen oxide emissions; Super-Ultra-Low-Emissions Vehicle II; downsizing AB Hydrogen is seen as a sustainable energy carrier for transportation because it can be generated using renewable energy sources and it is a favorable fuel for clean vehicle powertrains. Hydrogen internal-combustion engines have been identified as a cost-effective consumer of hydrogen in the near term to aid in the development of a large-scale hydrogen infrastructure. Current research on hydrogen internal-combustion engines is directed by a series of efficiency and emissions targets defined by the US Department of Energy including a peak brake thermal efficiency of 45% and nitrogen oxide emissions of less than 0.07 g/mile. A high-efficiency hydrogen direct-injection engine was developed at Argonne National Laboratory to take advantage of the combustion characteristics of hydrogen. The engine employs a lean control strategy with turbocharging for power density comparable with that of gasoline engines. The injection strategy was optimized through collaborative three-dimensional computational fluid dynamics and experimental efforts to achieve mixture stratification that is beneficial for both a high efficiency and low nitrogen oxide emissions. The efficiency maps of the hydrogen engine demonstrate a peak brake thermal efficiency of 45.5% together with nitrogen oxide maps showing emissions of less than 0.10 g/kW h in much of the operating regime. In order to evaluate the driving-cycle nitrogen oxide emissions, the engine maps were fed into a vehicle simulation assuming a midsize sedan with a conventional (non-hybrid) power-train. With a 3.0 l hydrogen engine, nitrogen oxide emissions from a Urban Dynamometer Driving Schedule cycle are 0.017 g/mile which fulfills the project goal and are even sufficiently low to meet the Super-Ultra-Low-Emissions Vehicle II emissions specification. The city or highway fuel economy, normalized to gallons of gasoline, is 32.4/51.5 mile/gal(US) for a combined average of 38.9 mile/gal(US), exceeding the 2016 Corporate Average Fuel Economy standard. Further vehicle simulations were performed to show the effect of engine downsizing. With a smaller 2.0 l engine, nitrogen oxide emissions increase to 0.028 g/mile, which still exceeds the US Department of Energy target together with the benefit of a fuel economy improvement to 45.4 mile/gal(US) (combined). C1 [Wallner, Thomas; Matthias, Nicholas S.; Scarcelli, Riccardo; Kwon, Jason C.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Wallner, T (reprint author), Argonne Natl Lab, Div Energy Syst, 9700 S Cass Ave, Argonne, IL 60439 USA. EM twallner@anl.gov FU Argonne, a U.S. Department of Energy Office of Science laboratory [DE-AC02-06CH11357]; DOE's FreedomCAR and Vehicle Technologies Program, Office of Energy Efficiency and Renewable Energy FX The submitted manuscript has been created by UChicago Argonne, LLC, Operator of Argonne National Laboratory ("Argonne"). Argonne, a U.S. Department of Energy Office of Science laboratory, is operated under Contract No. DE-AC02-06CH11357. The U. S. Government retains for itself, and others acting on its behalf, a paid-up nonexclusive, irrevocable worldwide license in said article to reproduce, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, by or on behalf of the Government.; This research was funded by DOE's FreedomCAR and Vehicle Technologies Program, Office of Energy Efficiency and Renewable Energy. The authors wish to thank Gurpreet Singh, program manager at DOE, for his support. The hydrogen engine used to run these experiments was provided by Ford Motor Company. Special thanks to Brad Boyer and his team from Ford Motor Company for their support. NR 23 TC 3 Z9 3 U1 0 U2 17 PU SAGE PUBLICATIONS LTD PI LONDON PA 1 OLIVERS YARD, 55 CITY ROAD, LONDON EC1Y 1SP, ENGLAND SN 0954-4070 J9 P I MECH ENG D-J AUT JI Proc. Inst. Mech. Eng. Part D-J. Automob. Eng. PY 2013 VL 227 IS 1 SI SI BP 99 EP 109 DI 10.1177/0954407012461875 PG 11 WC Engineering, Mechanical; Transportation Science & Technology SC Engineering; Transportation GA 114SM UT WOS:000316762700009 ER PT J AU Lee, H Rutland, CJ AF Lee, Hoon Rutland, Christopher J. TI Modeling uncontrolled regeneration of diesel particulate filters, taking into account hydrocarbon slip SO PROCEEDINGS OF THE INSTITUTION OF MECHANICAL ENGINEERS PART D-JOURNAL OF AUTOMOBILE ENGINEERING LA English DT Article DE Engine exhaust aftertreatment; diesel particulate filters; active regeneration; uncontrolled regeneration; hydrocarbon slip; numerical simulation ID OXIDATION AB The effect of hydrocarbon slip from a diesel oxidation catalyst on active regeneration of a diesel particulate filter is investigated by developing a generalized zero-dimensional diesel particulate filter model to predict the wall temperature of the diesel particulate filter and the trapped mass of particulate matter. Exhaust fuel injection methodology is applied to provide a high temperature for regeneration by oxidation in the diesel oxidation catalyst. However, the diesel oxidation catalyst reactions may be incomplete and hydrocarbon slip can occur. It is confirmed that two exothermic reactions, namely soot oxidation and hydrocarbon oxidation, which proceed simultaneously may result in the synergistic effect of a rise in the temperature. This is primarily because the temperature is the common factor that affects both reaction rates, i.e. a rise in the temperature caused by one reaction can affect the increase in the reaction rate of another reaction through the exotherms created. Accurate prediction of the temperature rise during active regeneration of the diesel particulate filter is dependent on several crucial factors: the initial wall temperature of the diesel particulate filter, the inlet temperature of the diesel particulate filter, the initial loading level of particulate matter, the exhaust mass flow rate, the oxygen concentration, and hydrocarbon slip. Several simulations revealed that hydrocarbon slip can be one of the reasons for uncontrolled regeneration of the diesel particulate filter. It is concluded that, if there is a considerable amount of hydrocarbon slip, then uncontrolled regeneration of the diesel particulate filter easily occurs when the exhaust mass flow rate is rapidly reduced to the idle condition during regeneration. Flow transient simulations also confirmed that the temperature ramp-up rate and the point of time when the exhaust mass flow rate is reduced determine the overall trend of the temperature rise and the characteristics of the thermal behavior of the diesel particulate filter. C1 [Lee, Hoon; Rutland, Christopher J.] Univ Wisconsin, Dept Mech Engn, Madison, WI 53706 USA. RP Lee, H (reprint author), Argonne Natl Lab, Div Energy Syst, Ctr Transportat Res, 9700 S Cass Ave, Argonne, IL 60439 USA. EM hoonlee@anl.gov NR 34 TC 1 Z9 1 U1 0 U2 18 PU SAGE PUBLICATIONS LTD PI LONDON PA 1 OLIVERS YARD, 55 CITY ROAD, LONDON EC1Y 1SP, ENGLAND SN 0954-4070 J9 P I MECH ENG D-J AUT JI Proc. Inst. Mech. Eng. Part D-J. Automob. Eng. PY 2013 VL 227 IS 2 BP 281 EP 296 DI 10.1177/0954407012450837 PG 16 WC Engineering, Mechanical; Transportation Science & Technology SC Engineering; Transportation GA 114TE UT WOS:000316764600012 ER PT J AU Xiang, Y Du, JC Skinner, LB Benmore, CJ Wren, AW Boydd, DJ Towler, MR AF Xiang, Ye Du, Jincheng Skinner, Lawrie B. Benmore, Chris J. Wren, Anthony W. Boydd, Daniel J. Towler, Mark R. TI Structure and diffusion of ZnO-SrO-CaO-Na2O-SiO2 bioactive glasses: a combined high energy X-ray diffraction and molecular dynamics simulations study SO RSC ADVANCES LA English DT Article ID ZINC-SILICATE-GLASSES; IN-VITRO; STRONTIUM SUBSTITUTION; FORCE-FIELDS; SODA-SILICA; ALUMINOPHOSPHATES; DIFFERENTIATION; SPECTROSCOPY; ENVIRONMENT; REACTIVITY AB Novel bioactive glasses that can release ions such as strontium and zinc provide bone growth enhancement and antibacterial properties that earlier-generation bioglasses did not possess. These glasses find applications in bone cementation, restoration and in tissue engineering. In this paper, we present combined experimental and simulation studies to explain the structure and diffusion of ZnO-SrO-CaO-Na2O-SiO2 bioactive glasses with the aim of understanding the short and medium range structure of these glasses, the structural correlation to their dissolution behaviors, and their bioactivity. High energy X-ray diffraction experiments have been performed to obtain structural information and to validate the structure models from simulations. Three glass compositions with ZnO/Na2O substitutions have been studied using molecular dynamics simulations to characterize the glass structure and calculate the ionic diffusion in these glasses. The results provide insight to local environments and structural role of zinc ions, the medium range structural features such as Q(n) distribution, and ionic diffusion characteristics of these bioactive glasses. The structure and ionic diffusion results are discussed in correlation to the dissolution behaviors and the bioactivity of these glasses. C1 [Xiang, Ye; Du, Jincheng] Univ N Texas, Dept Mat Sci & Engn, Denton, TX 76203 USA. [Skinner, Lawrie B.; Benmore, Chris J.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Wren, Anthony W.; Towler, Mark R.] Alfred Univ, Inamori Sch Engn, Alfred, NY 14802 USA. [Boydd, Daniel J.] Dalhousie Univ, Dept Appl Oral Sci Biomat & Oral Biol, Halifax, NS, Canada. [Towler, Mark R.] Ryerson Univ, Dept Mech & Ind Engn, Toronto, ON, Canada. [Towler, Mark R.] Univ Malaya, Dept Biomed Engn, Kuala Lumpur, Malaysia. [Skinner, Lawrie B.] SUNY Stony Brook, Dept Geosci, Stony Brook, NY 11794 USA. RP Xiang, Y (reprint author), Univ N Texas, Dept Mat Sci & Engn, Denton, TX 76203 USA. EM Jincheng.du@unt.edu RI Skinner, Lawrie/I-2603-2012; OI Skinner, Lawrie/0000-0001-7317-1642; Benmore, Chris/0000-0001-7007-7749 FU National Science Foundation (NSF) [0907593, 1105219]; US DOE [DE-FG02-09ER46650] FX JD acknowledges National Science Foundation (NSF) (#0907593 and #1105219) for financial support. LS was supported by US DOE grant DE-FG02-09ER46650. NR 57 TC 11 Z9 11 U1 4 U2 41 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2046-2069 J9 RSC ADV JI RSC Adv. PY 2013 VL 3 IS 17 BP 5966 EP 5978 DI 10.1039/c3ra23231j PG 13 WC Chemistry, Multidisciplinary SC Chemistry GA 117PO UT WOS:000316965800034 ER PT J AU Burr, T Hamada, MS AF Burr, T. Hamada, M. S. TI Revisiting Statistical Aspects of Nuclear Material Accounting SO SCIENCE AND TECHNOLOGY OF NUCLEAR INSTALLATIONS LA English DT Article AB Nuclear material accounting (NMA) is the only safeguards system whose benefits are routinely quantified. Process monitoring (PM) is another safeguards system that is increasingly used, and one challenge is how to quantify its benefit. This paper considers PM in the role of enabling frequent NMA, which is referred to as near-real-time accounting (NRTA). We quantify NRTA benefits using period-driven and data-driven testing. Period-driven testing makes a decision to alarm or not at fixed periods. Data-driven testing decides as the data arrives whether to alarm or continue testing. The difference between period-driven and datad-riven viewpoints is illustrated by using one-year and two-year periods. For both one-year and two-year periods, period-driven NMA using once-per-year cumulative material unaccounted for (CUMUF) testing is compared to more frequent Shewhart and joint sequential cusum testing using either MUF or standardized, independently transformed MUF (SITMUF) data. We show that the data-driven viewpoint is appropriate for NRTA and that it can be used to compare safeguards effectiveness. In addition to providing period-driven and data-driven viewpoints, new features include assessing the impact of uncertainty in the estimated covariance matrix of the MUF sequence and the impact of both random and systematic measurement errors. C1 [Burr, T.; Hamada, M. S.] Los Alamos Natl Lab, Stat Sci Grp, Los Alamos, NM 87545 USA. RP Burr, T (reprint author), Los Alamos Natl Lab, Stat Sci Grp, POB 1663, Los Alamos, NM 87545 USA. EM tburr@lanl.gov FU National Nuclear Security Administration Office of Nuclear Nonproliferation Research and Development program [NA-22]; Nuclear Energy (NE) program FX The authors acknowledge support from the National Nuclear Security Administration Office of Nuclear Nonproliferation Research and Development (NA-22) and Nuclear Energy (NE) programs. NR 25 TC 2 Z9 2 U1 0 U2 0 PU HINDAWI PUBLISHING CORPORATION PI NEW YORK PA 410 PARK AVENUE, 15TH FLOOR, #287 PMB, NEW YORK, NY 10022 USA SN 1687-6075 J9 SCI TECHNOL NUCL INS JI Sci. Technol. Nucl. Install. PY 2013 AR 961360 DI 10.1155/2013/961360 PG 15 WC Nuclear Science & Technology SC Nuclear Science & Technology GA 116RJ UT WOS:000316899900001 ER PT J AU Patra, L Messman, JM Toomey, R AF Patra, Leena Messman, Jamie M. Toomey, Ryan TI On the nature of volume-phase transitions in photo-cross-linked poly(cyclopropylacrylamide) and poly(N-vinylisobutyramide) coatings SO SOFT MATTER LA English DT Article ID SWELLING BEHAVIOR; AQUEOUS-SOLUTIONS; POLYMER NETWORKS; TEMPERATURE; FTIR; POLY(N-VINYLALKYLAMIDE); FUNCTIONALITIES; DERIVATIVES; HYDRATION; PROPERTY AB Ellipsometry in an inverted configuration was used to characterize the temperature-dependent swelling of thin (100 nm) coatings of photo-cross-linked poly(cyclopropylacrylamide), or poly(CPAAm), and poly(N-vinylisobutyramide), or poly(NVIBAm). Both polymers contained 3 mol% of methacroylaminobenzophenone (MnBP) as the photo-cross-linking unit. Poly(CPAAm-co-MnBP) showed a continuous, 2nd order deswelling transition between 10 and 70 degrees C with no hysteresis. Poly(NVIBAm-co-MnBP), on the other hand, showed a discontinuous, 1st order deswelling transition at 45 degrees C with a hysteresis in the swelling curve. The two types of swelling transitions are consistent with the cloud-point measurements of the uncross-linked polymers, which both showed lower-critical solution temperature (LCST) behavior. The LCST for poly(CPAAm-co-MnBP) is located at almost zero polymer concentration, and hence cross-linked poly(CPAAm) cannot cross its cloud point curve during swelling or deswelling. The LCST for poly(NVIBAm-co-MnBP), in contrast, is located at a significant off-zero polymer concentration (>10 wt% polymer), meaning cross-linked poly(NVIBAm) can cross its cloud point curve and experience a discontinuous jump in swelling. Concurrent measurements of the infrared vibrations of the amide groups in both systems further revealed that the amide I band in poly(CPAAm-co-MnBP) showed a single sub-band throughout the swelling transition. Poly(NVIBAm-co-MnBP), on the other hand, showed two distinct sub-bands, one of which grew at the expense of the other throughout the swelling transition, which may explain the off-zero concentration in the cloud point curve and the discontinuous swelling transition. C1 [Patra, Leena; Toomey, Ryan] Univ S Florida, Dept Chem & Biomed Engn, Tampa, FL 33620 USA. [Messman, Jamie M.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Toomey, R (reprint author), Univ S Florida, Dept Chem & Biomed Engn, Tampa, FL 33620 USA. EM toomey@usf.edu FU NSF [DMR-0645574]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX This work was supported by NSF DMR-0645574. Part of this research was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. NR 29 TC 2 Z9 2 U1 4 U2 18 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1744-683X J9 SOFT MATTER JI Soft Matter PY 2013 VL 9 IS 16 BP 4349 EP 4356 DI 10.1039/c3sm26962k PG 8 WC Chemistry, Physical; Materials Science, Multidisciplinary; Physics, Multidisciplinary; Polymer Science SC Chemistry; Materials Science; Physics; Polymer Science GA 117LQ UT WOS:000316955300023 ER PT J AU Swensen, JS Wang, L Polikarpov, E Rainbolt, JE Koech, PK Cosimbescu, L Padmaperuma, AB AF Swensen, James S. Wang, Liang Polikarpov, Evgueni Rainbolt, James E. Koech, Phillip K. Cosimbescu, Lelia Padmaperuma, Asanga B. TI Near independence of OLED operating voltage on transport layer thickness SO SYNTHETIC METALS LA English DT Article DE F3TCNQ-Adl; OLEDs; Conductivity doping; Injection barriers; Blue OLEDs ID ORGANIC ELECTROLUMINESCENT DEVICES; LIGHT-EMITTING-DIODES; INDIUM-TIN-OXIDE; ELECTRONIC DEVICES; WORK FUNCTION; EFFICIENCY; INJECTION AB We report organic light emitting devices (OLEDs) with weak drive voltage dependence on the thickness of the hole transport layer (HTL) for thicknesses up to 1150 angstrom using the N,N'-Bis(naphthalen-1-yl)-N,N'-bis(phenyl)-benzidine (alpha-NPD) and N,N'-bis(3-methyl phenyl)-N,N'-diphenyl-[1,1'-biphenyl]-4,4'diamine (TPD), both of which have hole mobilities in the range of 2 x 10(-3) cm(2) V-1 s(-1). Lower mobility HTL materials show larger operating voltage dependence on thickness. The near independence of the operating voltage for high mobility transport material thickness was only observed when the energy barrier for charge injection into the transport material was minimized. To ensure low injection barriers, a thin film of 2-(3-(adamantan-1-yl)propyl)-3,5,6-trifluorotetracyanoquinodimethane (F3TCNQ-Adl) was cast from solution onto the ITO surface. These results indicate that thick transport layers can be integrated into OLED stacks without the need for bulk conductivity doping, potentially reducing device and material complexity and lowering overall cost. (C) 2013 Published by Elsevier B.V. C1 [Swensen, James S.; Wang, Liang; Polikarpov, Evgueni; Rainbolt, James E.; Koech, Phillip K.; Cosimbescu, Lelia; Padmaperuma, Asanga B.] Pacific NW Natl Lab, Appl Mat Sci Grp, Richland, WA 99352 USA. RP Padmaperuma, AB (reprint author), Pacific NW Natl Lab, 902 Battelle Blvd,POB 999,MSIN K2-44, Richland, WA 99352 USA. EM asanga.padmaperuma@pnl.gov OI Koech, Phillip/0000-0003-2996-0593 FU Solid State Lighting Program of the U.S. Department of Energy (US DOE), within the Building Technologies Program (BT) [M6743231, M68004043]; U.S. DOE [DE_AC06-76RLO 1830] FX This project was funded by the Solid State Lighting Program of the U.S. Department of Energy (US DOE), within the Building Technologies Program (BT) (Award Nos. M6743231 and M68004043, managed by the National Energy Technology Laboratory (NETL)). Pacific Northwest National Laboratory (PNNL) is operated by Battelle Memorial Institute for the U.S. DOE (under Contract DE_AC06-76RLO 1830). NR 20 TC 1 Z9 1 U1 2 U2 42 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0379-6779 J9 SYNTHETIC MET JI Synth. Met. PD JAN 1 PY 2013 VL 163 BP 29 EP 32 DI 10.1016/j.synthmet.2012.12.015 PG 4 WC Materials Science, Multidisciplinary; Physics, Condensed Matter; Polymer Science SC Materials Science; Physics; Polymer Science GA 113DN UT WOS:000316646800006 ER PT S AU Ferreira, JA Braga, MH AF Ferreira, J. A. Braga, M. H. BE Pinto, AMP Pouzada, AS TI First Principles Study of Copper Sulfides (for applications as photoconductors) SO ADVANCED MATERIALS FORUM VI, PTS 1 AND 2 SE Materials Science Forum LA English DT Proceedings Paper CT 6th International Materials Symposium (MATERIALS 2011)/15th Meeting of SPM CY APR 18-20, 2011 CL Univ Minho, Guimaraes, PORTUGAL SP Portuguese Mat Soc, Univ Minho, Sch Engn, Portuguese Fdn Sci & Technol, Ctr Mech & Mat Technol, Inst Polym & Composites, 3Bs Res Grp Biomaterials Biodegradables & Biomimet, Minho Univ, Ctr Phys, Um, Sch Sci, TecMinho, Town Hall Guimaraes, Beneq, Celoplas, Filsat, Izasa, Leica MicroSystems, Mario Costa Martins & Filho Lda, Panalytical, ScienTec HO Univ Minho DE Band Structures; Mechanical Properties; Sulfides; Photovoltaics ID AUGMENTED-WAVE METHOD AB The Tetrahedrite's family constitutes a complete solid-solution series, and is among the most frequent complex sulfides in Nature. This kind of structure can be generically expressed by the composition, Cu12Sb4S13. We have calculated the electronic band structure of Cu12Sb4S13 and Ag6Cu6Sb4S13 (with band gaps of 1.24 and 1.20 eV, respectively) to demonstrate that different elements occupying certain sites of the crystal structure will make a difference in what concerns the conduction process in Tetrahedrites. We will use this effect and ab initio calculations to show that the electronic properties of these compounds make them promising candidates as solar cells photovoltaic materials since not only they possess a direct band gap but their energy falls within the range of energies of photovoltaics. Moreover, we can optimize these properties by doping and substituting ions furthermore. Mechanical properties were also calculated for both compounds and will be compared. C1 [Ferreira, J. A.] LNEG, Sao Mamede de Infesta, Portugal. [Braga, M. H.] Los Alamos Neutron Scattering Ctr, Los Alamos Natl Lab, Los Alamos, NM USA. [Braga, M. H.] Univ Porto, Fac Engn, CEMUC, Engn Phys Dep, Oporto, Portugal. RP Ferreira, JA (reprint author), LNEG, Sao Mamede de Infesta, Portugal. EM jorge.ferreira@lneg.pt; mbraga@fe.up.pt RI LNEG, Producao Cientifica/D-2212-2012; Braga, Maria Helena/A-2491-2014; Ferreira, J. Jorge/M-5209-2015 OI Braga, Maria Helena/0000-0003-4577-2154; NR 14 TC 1 Z9 1 U1 0 U2 20 PU TRANS TECH PUBLICATIONS LTD PI DURNTEN-ZURICH PA KREUZSTRASSE 10, 8635 DURNTEN-ZURICH, SWITZERLAND SN 0255-5476 J9 MATER SCI FORUM PY 2013 VL 730-732 BP 111 EP + DI 10.4028/www.scientific.net/MSF.730-732.111 PG 2 WC Materials Science, Multidisciplinary SC Materials Science GA BDX70 UT WOS:000315545200019 ER PT S AU Braga, MH Sa, MN Ferreira, JA Daemen, LL AF Braga, M. H. Sa, M. N. Ferreira, J. A. Daemen, L. L. BE Pinto, AMP Pouzada, AS TI First Principles Calculations and Experiments to Determine the Hydrogenation Process of Cu-Li-Mg SO ADVANCED MATERIALS FORUM VI, PTS 1 AND 2 SE Materials Science Forum LA English DT Proceedings Paper CT 6th International Materials Symposium (MATERIALS 2011)/15th Meeting of SPM CY APR 18-20, 2011 CL Univ Minho, Guimaraes, PORTUGAL SP Portuguese Mat Soc, Univ Minho, Sch Engn, Portuguese Fdn Sci & Technol, Ctr Mech & Mat Technol, Inst Polym & Composites, 3Bs Res Grp Biomaterials Biodegradables & Biomimet, Minho Univ, Ctr Phys, Um, Sch Sci, TecMinho, Town Hall Guimaraes, Beneq, Celoplas, Filsat, Izasa, Leica MicroSystems, Mario Costa Martins & Filho Lda, Panalytical, ScienTec HO Univ Minho DE Cu-Li-Mg-H; Density Functional Theory (DFT); Phonons; Neutron Scattering ID INELASTIC NEUTRON-SCATTERING; AUGMENTED-WAVE METHOD; STORAGE PROPERTIES; MAGNESIUM HYDRIDE AB Density Functional Theory (DFT) calculations were performed. They were firstly implemented to optimize the structure and refine the stoichiometry of the only ternary compound, CuLi0.08Mg1.92 of the Cu-Li-Mg system. Furthermore using DFT, several possible structures of CuMg2Hx were optimized. Since most of the hydrides are cubic structures or can be considered as distortions of a cubic structure, we have started calculations for CuMg2Hx (x = 4 - 6) with tetragonal and monoclinic structures, similar to those of the hydrides formed by the nearest neighbors of Cu and Mg in the periodic table: NiMg2H4 and CoMg2H5 (e.g. monoclinic C2/c and tetragonal P4/nmm, respectively). It can be concluded that the most stable configuration corresponds to CuMg2H5 with C2/c structure. We have performed several neutron scattering experiments that are in agreement with the first principles calculations. C1 [Braga, M. H.; Daemen, L. L.] Los Alamos Natl Lab, Los Alamos Neutron Scattering Ctr, Los Alamos, NM 87545 USA. [Braga, M. H.; Sa, M. N.] Univ Porto, Fac Engn, CEMUC, Engn Phys Dep, Oporto, Portugal. [Ferreira, J. A.] LNEG Lab Nacl Energia Geol, Amadora, Portugal. RP Braga, MH (reprint author), Los Alamos Natl Lab, Los Alamos Neutron Scattering Ctr, Los Alamos, NM 87545 USA. EM mbraga@fe.up.pt; mhsa@fe.up.pt; jorge.ferreira@lneg.pt; lld@lanl.gov RI Braga, Maria Helena/A-2491-2014; Ferreira, J. Jorge/M-5209-2015 OI Braga, Maria Helena/0000-0003-4577-2154; FU FCT [PTDC/CTM/099461/2008, FCOMP-01-0124-FEDER-009369]; DOE Office of Basic Energy Sciences, USA FX The authors would like to acknowledge Portuguese Science Foundation, FCT, for the project (PTDC/CTM/099461/2008 and and FCOMP-01-0124-FEDER-009369). This work has benefited from the use of neutron scattering instruments NPDF, HIPD and FDS at the Lujan Center at Los Alamos Neutron Science Center, funded by DOE Office of Basic Energy Sciences, USA. This work has benefited from the use of 11-beamline at the Advanced Photon Source at Argonne National Laboratory, USA. NR 19 TC 0 Z9 0 U1 0 U2 4 PU TRANS TECH PUBLICATIONS LTD PI DURNTEN-ZURICH PA KREUZSTRASSE 10, 8635 DURNTEN-ZURICH, SWITZERLAND SN 0255-5476 J9 MATER SCI FORUM PY 2013 VL 730-732 BP 799 EP + DI 10.4028/www.scientific.net/MSF.730-732.799 PG 2 WC Materials Science, Multidisciplinary SC Materials Science GA BDX70 UT WOS:000315545200132 ER PT J AU James, JZ Lucas, D Koshland, CP AF James, Jay Z. Lucas, Donald Koshland, Catherine P. TI Elemental mercury vapor interaction with individual gold nanorods SO ANALYST LA English DT Article ID SURFACE-PLASMON RESONANCE; SILVER NANOPARTICLES; ASPECT RATIO; SINGLE GOLD; FILMS; ABSORPTION; ADSORPTION; SPECTROSCOPY; QUANTITIES; SENSORS AB We show that single gold nanorods can act as highly sensitive mercury vapor sensors with attogram resolution. We exposed assorted gold nanorods, with aspect ratios ranging from 2.8-4.1, to mu g m(-3) concentrations of mercury vapor in air for 1 hour. Pre- and post-exposure, the nanorods were examined with a combination of dark field spectroscopy and transmission electron microscopy. Because we isolated individual particles, we can describe the shape and size effects distinctly rather than statistically (a constraint of studying heterogeneous nanoparticle films). No measurable changes occurred to the shape and size of the nanorods due to their saturation with mercury vapor. The localized surface plasmon resonance (LSPR) of the mercury-saturated nanorods blue shifted 2.6-3.8 nm; the magnitude of the shift depended on the initial shape and size of the nanorod. Larger aspect ratios and surface-area-to-volume ratios both enhance the LSPR shift seen in saturated nanoparticles. The predictions of a core-shell model mirrors the shape and size effects observed experimentally. These results increase our understanding of mercury-adsorption by gold surfaces, and help to optimize nanoparticle-based plasmonic mercury sensing. C1 [James, Jay Z.] Univ Calif Berkeley, Dept Mech Engn, Berkeley, CA 94720 USA. [Lucas, Donald] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Koshland, Catherine P.] Univ Calif Berkeley, Sch Publ Hlth, Berkeley, CA 94720 USA. RP James, JZ (reprint author), Univ Calif Berkeley, Dept Mech Engn, Berkeley, CA 94720 USA. EM jayjames@berkeley.edu NR 32 TC 12 Z9 12 U1 3 U2 40 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 0003-2654 J9 ANALYST JI Analyst PY 2013 VL 138 IS 8 BP 2323 EP 2328 DI 10.1039/c3an36841f PG 6 WC Chemistry, Analytical SC Chemistry GA 107MS UT WOS:000316222300015 PM 23446550 ER PT J AU Guo, SJ Li, DG Zhu, HY Zhang, S Markovic, NM Stamenkovic, VR Sun, SH AF Guo, Shaojun Li, Dongguo Zhu, Huiyuan Zhang, Sen Markovic, Nenad M. Stamenkovic, Vojislav R. Sun, Shouheng TI FePt and CoPt Nanowires as Efficient Catalysts for the Oxygen Reduction Reaction SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE alloys; heterogeneous catalysis; nanostructures; oxygen reduction reaction; platinum ID PT-SKIN SURFACES; FUEL-CELLS; ELECTROCATALYSTS; NANOPARTICLES; GRAPHENE; NANOCRYSTALS; BATTERIES; OXIDATION; ULTRATHIN; DESIGN C1 [Guo, Shaojun; Li, Dongguo; Zhu, Huiyuan; Zhang, Sen; Sun, Shouheng] Brown Univ, Dept Chem, Providence, RI 02912 USA. [Li, Dongguo; Markovic, Nenad M.; Stamenkovic, Vojislav R.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Stamenkovic, VR (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM vrstamenkovic@anl.gov; ssun@brown.edu RI Guo, Shaojun/A-8449-2011; Zhang, Sen/E-4226-2015; Li, Dongguo/O-6253-2016 OI Guo, Shaojun/0000-0002-5941-414X; Li, Dongguo/0000-0001-7578-7811 FU U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Fuel Cell Technologies Program FX Supported by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Fuel Cell Technologies Program. NR 35 TC 163 Z9 166 U1 43 U2 507 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PY 2013 VL 52 IS 12 BP 3465 EP 3468 DI 10.1002/anie.201209871 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA 109CN UT WOS:000316342900032 PM 23420804 ER PT J AU Alonso, DM Gallo, JMR Mellmer, MA Wettstein, SG Dumesic, JA AF Alonso, David Martin Gallo, Jean Marcel R. Mellmer, Max A. Wettstein, Stephanie G. Dumesic, James A. TI Direct conversion of cellulose to levulinic acid and gamma-valerolactone using solid acid catalysts SO CATALYSIS SCIENCE & TECHNOLOGY LA English DT Article ID ZEOLITE CATALYST; BIOMASS; GLUCOSE; LIQUID; FUELS; DECOMPOSITION; HYDROGENATION; DEHYDRATION; CHEMICALS; FRUCTOSE AB Cellulose was converted with high yield (69%) to levulinic acid (LA) using Amberlyst 70 as the catalyst and using a solution of 90 wt% gamma-valerolactone (GVL) and 10 wt% water as the solvent, compared to the low yield of 20% obtained in water. The LA was upgraded to GVL without any neutralization or purification steps due to the solubilization of humins by the GVL solvent. High LA yields (54%) were also obtained from real biomass (corn stover). C1 [Alonso, David Martin; Gallo, Jean Marcel R.; Mellmer, Max A.; Wettstein, Stephanie G.; Dumesic, James A.] Univ Wisconsin, Dept Chem & Biol Engn, Madison, WI 53706 USA. [Mellmer, Max A.; Wettstein, Stephanie G.; Dumesic, James A.] Univ Wisconsin, DOE Great Lakes Bioenergy Res Ctr, Madison, WI 53706 USA. RP Alonso, DM (reprint author), Univ Wisconsin, Dept Chem & Biol Engn, 1415 Engn Dr, Madison, WI 53706 USA. EM dumesic@engr.wisc.edu RI Gallo, Jean Marcel/C-9985-2013 OI Gallo, Jean Marcel/0000-0003-2937-2628 FU Defense Advanced Research Projects Agency; DOE Great Lakes Bioenergy Research Center [BER DE-FC02-07ER64494]; DOE FX This work was supported through funding from the Defense Advanced Research Projects Agency (Surf-cat: Catalysts for Production of JP-8 range molecules from Lignocellulosic Biomass).The views, opinions, and/or findings contained in this article are those of the author and should not be interpreted as representing the official views or policies, either expressed or implied, of the Defense Advanced Research Projects Agency or the Department of Defense. In addition this work was funded in part by the DOE Great Lakes Bioenergy Research Center (DOE Office of Science BER DE-FC02-07ER64494) and the DOE. The authors would like to thank Jher Hau Yeap and Hui Chin Wong for helping with the experiments reported in this paper. NR 36 TC 66 Z9 69 U1 10 U2 225 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2044-4753 J9 CATAL SCI TECHNOL JI Catal. Sci. Technol. PY 2013 VL 3 IS 4 BP 927 EP 931 DI 10.1039/c2cy20689g PG 5 WC Chemistry, Physical SC Chemistry GA 103MF UT WOS:000315920300006 ER PT J AU Buckley, HL Anstey, MR Gryko, DT Arnold, J AF Buckley, Heather L. Anstey, Mitchell R. Gryko, Daniel T. Arnold, John TI Lanthanide corroles: a new class of macrocyclic lanthanide complexes SO CHEMICAL COMMUNICATIONS LA English DT Article ID PORPHYRIN COMPLEXES; METAL-COMPLEXES; CHEMISTRY; IONS; 5,10,15-TRIS(PENTAFLUOROPHENYL)CORROLE; LUMINESCENCE; LIGANDS; REAGENT; PROBES; CERIUM AB The first examples of lanthanide corroles are prepared by two synthetic routes. (Mes(2)(p-OMePh)corrole)La center dot 4.5DME (1 center dot 4.5DME) and (Mes(2)(p-OMePh)corrole) Tb center dot 4DME (2 center dot 4DME) are prepared from the free base corrole and Ln((NSiMe3)(2))(3), while (Mes(2)(p-OMePh)corrole)-Gd center dot TACNMe(3) (3 center dot TACNMe(3)) is prepared by metathesis of the recently reported Li-3 corrole and GdCl3. C1 [Buckley, Heather L.; Arnold, John] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Anstey, Mitchell R.] Sandia Natl Labs, Livermore, CA 94550 USA. [Gryko, Daniel T.] Polish Acad Sci, Inst Organ Chem, Warsaw, Poland. [Gryko, Daniel T.] Warsaw Univ Technol, Fac Chem, Warsaw, Poland. RP Anstey, MR (reprint author), Sandia Natl Labs, Livermore, CA 94550 USA. EM mantsey@sandia.gov; dtgryko@icho.edu.pl; arnold@berkeley.edu RI Gryko, Daniel/A-7998-2008; Arnold, John/F-3963-2012 OI Gryko, Daniel/0000-0002-2146-1282; Arnold, John/0000-0001-9671-227X FU International Fulbright Science and Technology Fellowship; United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; EUROCORES Programme EuroSolarFuels (Polish National Science Centre) FX HLB acknowledges the International Fulbright Science and Technology Fellowship. MRA thanks the Laboratory Directed Research and Development Program at Sandia National Laboratories. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL85000. DTG thanks EUROCORES Programme EuroSolarFuels (Polish National Science Centre). We are grateful to Antonio DiPasquale (XRD), Zhongrui Zhou (MS), and Olivia Lee (NMR) for assistance with instrumentation. NR 40 TC 24 Z9 24 U1 0 U2 63 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1359-7345 J9 CHEM COMMUN JI Chem. Commun. PY 2013 VL 49 IS 30 BP 3104 EP 3106 DI 10.1039/c3cc38806a PG 3 WC Chemistry, Multidisciplinary SC Chemistry GA 108EM UT WOS:000316274500005 PM 23467462 ER PT J AU Lindsay, AM Galloway-Carson, M Johnson, CR Bunde, DP Leung, VJ AF Lindsay, A. M. Galloway-Carson, M. Johnson, C. R. Bunde, D. P. Leung, V. J. TI Backfilling with guarantees made as jobs arrive SO CONCURRENCY AND COMPUTATION-PRACTICE & EXPERIENCE LA English DT Article DE parallel job scheduling; backfilling ID PERFORMANCE; PREDICTIONS AB In this paper, we present scheduling algorithms that simultaneously support guaranteed starting times and favor jobs with system-desired traits. To achieve the first of these goals, our algorithms keep a profile with potential starting times for every unfinished job and never move these starting times later, just as in Conservative Backfilling. To achieve the second, they exploit previously unrecognized flexibility in the handling of holes opened in this profile when jobs finish early. We find that, with one choice of job selection function, our algorithms can consistently reduce average waiting time and average bounded slowdown relative to Conservative Backfilling while still providing a guaranteed start time to each job as it arrives. In fact, in most cases, the algorithms give better performance than the more aggressive Extensible Argonne Scheduling System (EASY) backfilling algorithm, which does not provide guaranteed start times. Alternately, with a different choice of job selection function, our algorithms can focus the benefit on the widest submitted jobs, the reason for the existence of parallel systems. In this case, these jobs experience significantly lower waiting times than Conservative Backfilling with minimal impact on other jobs. Copyright (C) 2012 John Wiley & Sons, Ltd. C1 [Lindsay, A. M.] IBASEt, Foothill Ranch, CA USA. [Galloway-Carson, M.; Bunde, D. P.] Knox Coll, Galesburg, IL 61401 USA. [Johnson, C. R.] MIT, Cambridge, MA 02139 USA. [Leung, V. J.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Bunde, DP (reprint author), Knox Coll, 2 E South St, Galesburg, IL 61401 USA. EM dbunde@knox.edu FU Sandia National Laboratories [763836, 899808]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was carried out while A. M. Lindsay and C. R. Johnson were students at Knox College. A. M. Lindsay, M. Galloway-Carson, C. R. Johnson, and D. P. Bunde were partially supported by contracts 763836 and 899808 from Sandia National Laboratories. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 19 TC 3 Z9 3 U1 0 U2 2 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1532-0626 J9 CONCURR COMP-PRACT E JI Concurr. Comput.-Pract. Exp. PY 2013 VL 25 IS 4 SI SI BP 513 EP 523 DI 10.1002/cpe.2860 PG 11 WC Computer Science, Software Engineering; Computer Science, Theory & Methods SC Computer Science GA 107PQ UT WOS:000316230900008 ER PT J AU Lakshminarasimhan, S Shah, N Ethier, S Ku, SH Chang, CS Klasky, S Latham, R Ross, R Samatova, NF AF Lakshminarasimhan, Sriram Shah, Neil Ethier, Stephane Ku, Seung-Hoe Chang, C. S. Klasky, Scott Latham, Rob Ross, Rob Samatova, Nagiza F. TI ISABELA for effective in situ compression of scientific data SO CONCURRENCY AND COMPUTATION-PRACTICE & EXPERIENCE LA English DT Article DE lossy compression; B-spline; in situ processing; data-intensive application; high performance computing ID FLOATING-POINT DATA; LOSSLESS COMPRESSION; B-SPLINES AB Exploding dataset sizes from extreme-scale scientific simulations necessitates efficient data management and reduction schemes to mitigate I/O costs. With the discrepancy between I/O bandwidth and computational power, scientists are forced to capture data infrequently, thereby making data collection an inherently lossy process. Although data compression can be an effective solution, the random nature of real-valued scientific datasets renders lossless compression routines ineffective. These techniques also impose significant overhead during decompression, making them unsuitable for data analysis and visualization, which require repeated data access. To address this problem, we propose an effective method for In situ Sort-And-B-spline Error-bounded Lossy Abatement (ISABELA) of scientific data that is widely regarded as effectively incompressible. With ISABELA, we apply a pre-conditioner to seemingly random and noisy data along spatial resolution to achieve an accurate fitting model that guarantees a >= 0.99 correlation with the original data. We further take advantage of temporal patterns in scientific data to compress data by approximate to 85%, while introducing only a negligible overhead on simulations in terms of runtime. ISABELA significantly outperforms existing lossy compression methods, such as wavelet compression, in terms of data reduction and accuracy. We extend upon our previous paper by additionally building a communication-free, scalable parallel storage framework on top of ISABELA-compressed data that is ideally suited for extreme-scale analytical processing. The basis for our storage framework is an inherently local decompression method (it need not decode the entire data), which allows for random access decompression and low-overhead task division that can be exploited over heterogeneous architectures. Furthermore, analytical operations such as correlation and query processing run quickly and accurately over data in the compressed space. Copyright (C) 2012 John Wiley & Sons, Ltd. C1 [Lakshminarasimhan, Sriram; Shah, Neil; Samatova, Nagiza F.] N Carolina State Univ, Raleigh, NC 27695 USA. [Lakshminarasimhan, Sriram; Klasky, Scott; Samatova, Nagiza F.] Oak Ridge Natl Lab, Oak Ridge, TN 37830 USA. [Ethier, Stephane; Ku, Seung-Hoe; Chang, C. S.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. [Latham, Rob; Ross, Rob] Argonne Natl Lab, Argonne, IL 60439 USA. RP Samatova, NF (reprint author), N Carolina State Univ, Raleigh, NC 27695 USA. EM samatova@csc.ncsu.edu RI Ku, Seung-Hoe/D-2315-2009 OI Ku, Seung-Hoe/0000-0002-9964-1208 FU US Department of Energy, Office of Science; US National Science Foundation (Expeditions in Computing); LLC U.S. D.O.E. [DEAC05-00OR22725] FX We would like to thank ORNLs and ANLs leadership class computing facilities, OLCF and ALCF respectively, for the use of their resources. We would also like to acknowledge the use of those scientific datasets at Flash Center for Computational Science. Additionally, we would like to thank the development teams of the XGC1 and GTS simulations for the data used in this paper. This work was supported in part by the US Department of Energy, Office of Science and the US National Science Foundation (Expeditions in Computing). Oak Ridge National Laboratory is managed by UT-Battelle for the LLC U.S. D.O.E. under contract no. DEAC05-00OR22725. NR 24 TC 6 Z9 7 U1 0 U2 23 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1532-0626 J9 CONCURR COMP-PRACT E JI Concurr. Comput.-Pract. Exp. PY 2013 VL 25 IS 4 SI SI BP 524 EP 540 DI 10.1002/cpe.2887 PG 17 WC Computer Science, Software Engineering; Computer Science, Theory & Methods SC Computer Science GA 107PQ UT WOS:000316230900009 ER PT J AU Poineau, F Weck, PF Burton-Pye, BP Denden, I Kim, E Kerlin, W German, KE Fattahi, M Francesconi, LC Sattelberger, AP Czerwinski, KR AF Poineau, Frederic Weck, Philippe F. Burton-Pye, Benjamin P. Denden, Ibthihel Kim, Eunja Kerlin, William German, Konstantin E. Fattahi, Massoud Francesconi, Lynn C. Sattelberger, Alfred P. Czerwinski, Kenneth R. TI Reactivity of HTcO4 with methanol in sulfuric acid: Tc-sulfate complexes revealed by XAFS spectroscopy and first principles calculations SO DALTON TRANSACTIONS LA English DT Article ID RAY-ABSORPTION SPECTROSCOPY; CHEMISTRY; PERMANGANATE; OXIDATION; ALCOHOLS; ETHANOL; WATER; ION AB The reaction between HTcO4 and MeOH in 13 M H2SO4 was investigated by Tc-99 NMR, UV-visible and X-ray absorption fine structure (XAFS) spectroscopy. Experimental results and first principles calculations show the formation of Tc(+5) sulfate complexes. The results expand the fundamental understanding of Tc in high acid solutions. C1 [Poineau, Frederic; Kerlin, William; Czerwinski, Kenneth R.] Univ Nevada, Dept Chem, Las Vegas, NV 89154 USA. [Weck, Philippe F.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Burton-Pye, Benjamin P.; Francesconi, Lynn C.] CUNY Hunter Coll, Dept Chem, New York, NY 10065 USA. [Denden, Ibthihel; Fattahi, Massoud] Ecoles Mines Nantes, Lab Subatech, Nantes 44, France. [Kim, Eunja] Univ Nevada, Dept Phys & Astron, Las Vegas, NV 89154 USA. [German, Konstantin E.] Russian Acad Sci, AN Frumkin Inst Phys Chem & Electrochem, Moscow 119071, Russia. [Sattelberger, Alfred P.] Argonne Natl Lab, Energy Engn & Syst Anal Directorate, Lemont, IL 60439 USA. RP Poineau, F (reprint author), Univ Nevada, Dept Chem, Las Vegas, NV 89154 USA. EM poineauf@unlv.nevada.edu RI German, Konstantin/B-7694-2011; OI German, Konstantin/0000-0003-2368-4081; , Philippe/0000-0002-7610-2893 FU NEUP grant "Development of Alternative Technetium Waste Forms" from the U.S. Department of Energy, Office of Nuclear Energy, through INL/BEA, LLC [89445]; NSF-IGERT through Hunter College [40A70-A/01010670]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; SISGR, Heavy Element Chemistry, Office of Science, Department of Energy [DE-FG02-09ER16097]; [NSF-CHE-0959617]; [NSF-CHE-0750118] FX Funding for this research was provided by an NEUP grant "Development of Alternative Technetium Waste Forms" from the U.S. Department of Energy, Office of Nuclear Energy, through INL/BEA, LLC, 89445. Further support was provided by NSF-IGERT contract 40A70-A/01010670 through Hunter College. Use of the Advanced Photon Source at Argonne was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC0-206CH11357. Sandia National Laboratories is a multiprogram laboratory operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Company, for the United States Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL85000. The work conducted at Hunter College was supported by NSF-CHE-0959617 (for purchase of the 400 MHz NMR spectrometer), NSF-CHE-0750118, and DE-FG02-09ER16097 (SISGR, Heavy Element Chemistry, Office of Science, Department of Energy). The authors thank Trevor Low, and Julie Bertoia for outstanding health physics support and Dr Sungsik Lee at the APS for support during the EXAFS experiment. NR 24 TC 8 Z9 8 U1 1 U2 24 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1477-9226 EI 1477-9234 J9 DALTON T JI Dalton Trans. PY 2013 VL 42 IS 13 BP 4348 EP 4352 DI 10.1039/c3dt32951h PG 5 WC Chemistry, Inorganic & Nuclear SC Chemistry GA 108LK UT WOS:000316294400004 PM 23403900 ER PT J AU Weck, PF Kim, E Jove-Colon, CF Sassani, DC AF Weck, Philippe F. Kim, Eunja Jove-Colon, Carlos F. Sassani, David C. TI On the role of strong electron correlations in the surface properties and chemistry of uranium dioxide SO DALTON TRANSACTIONS LA English DT Article ID BRILLOUIN-ZONE INTEGRATIONS; ACTINIDE OXIDE SURFACES; AUGMENTED-WAVE METHOD; MEAN-FIELD THEORY; SINGLE-CRYSTAL; CORRELATION-ENERGY; UO2 SURFACES; DENSITY; 1ST-PRINCIPLES; SPECTRA AB We report density functional calculations of the surface properties and chemistry of UO2(111) performed within the generalized gradient approximation corrected with an effective Hubbard parameter (GGA + U within Dudarev's formalism) to account for the strong on-site Coulomb repulsion between U 5f electrons. The variation of the properties of periodic slab models, with collinear ferromagnetic and antiferromagnetic arrangements of the uranium magnetic moments, was investigated while ramping up the effective Hubbard parameter from U-eff = 0 eV, corresponding to standard density functional theory, up to U-eff = 4 eV, the value that correctly reproduces the antiferromagnetic ground state of bulk UO2. The chemical interactions of molecular water, dissociated water, dissociated oxygen and co-adsorbed molecular water and monatomic oxygen with the UO2(111) surface were also studied as functions of the U-eff parameter. Calculations reveal that some of the key electronic and chemical properties controlling the surface reactivity are very sensitive to the value of this strong electron correlation parameter. C1 [Weck, Philippe F.; Jove-Colon, Carlos F.; Sassani, David C.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Kim, Eunja] Univ Nevada, Dept Phys & Astron, Las Vegas, NV 89154 USA. RP Weck, PF (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM pfweck@sandia.gov OI , Philippe/0000-0002-7610-2893 FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; Used Fuel Disposition Campaign of the U. S. Department of Energy's Office of Nuclear Energy FX Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. Funding for this work was provided by the Used Fuel Disposition Campaign of the U. S. Department of Energy's Office of Nuclear Energy. We thank Alexander Thompson and Christopher Wolverton (Northwestern University) for providing us with the optimized structure of uranium dioxide with distortion of the oxygen sublattice, as well as Frances Smith-Skomurski (Pacific Northwest National Laboratory) and Udo Becker (U. MichiganAnn Arbor) for the structures of their surface models optimized with standard DFT. NR 69 TC 12 Z9 13 U1 3 U2 40 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1477-9226 J9 DALTON T JI Dalton Trans. PY 2013 VL 42 IS 13 BP 4570 EP 4578 DI 10.1039/c3dt32536a PG 9 WC Chemistry, Inorganic & Nuclear SC Chemistry GA 108LK UT WOS:000316294400032 PM 23354003 ER PT J AU Vasudevan, KV Smythe, NC Scott, BL Gordon, JC AF Vasudevan, Kalyan V. Smythe, Nathan C. Scott, Brian L. Gordon, John C. TI Metallopolymer formation using the (1R,2R)-N,N '-bis(pyridylmethylene)cyclohexane-1,2-diamine (BPID) ligand class SO DALTON TRANSACTIONS LA English DT Article ID COMPLEXES; CRYSTAL; METAL; POLYMERS; SODIUM AB The BPID ligand class is exploited as a scaffold for polymeric materials. Reaction of excess K or KH with the 2-pyridyl-BPID ligand results in the formation of a novel THF-bridged 1-D metallopolymer while the analogous reaction with the 4-pyridyl derivative results in a pyridyl-bridged 2-D metallopolymer. C1 [Vasudevan, Kalyan V.; Smythe, Nathan C.; Gordon, John C.] Los Alamos Natl Lab, Div Chem, Los Alamos, NM 87545 USA. [Scott, Brian L.] Los Alamos Natl Lab, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA. RP Gordon, JC (reprint author), Los Alamos Natl Lab, Div Chem, POB 1663, Los Alamos, NM 87545 USA. EM jgordon@lanl.gov RI Scott, Brian/D-8995-2017 OI Scott, Brian/0000-0003-0468-5396 NR 22 TC 0 Z9 0 U1 2 U2 13 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1477-9226 J9 DALTON T JI Dalton Trans. PY 2013 VL 42 IS 14 BP 4768 EP 4771 DI 10.1039/c3dt50327e PG 4 WC Chemistry, Inorganic & Nuclear SC Chemistry GA 108LU UT WOS:000316295500003 PM 23426568 ER PT J AU Galiano, V Lopez-Granado, O Malumbres, MP Drummond, LA Migallon, H AF Galiano, Vicente Lopez-Granado, Otoniel Malumbres, Manuel P. Drummond, Leroy Anthony Migallon, Hector TI GPU-based 3D lower tree wavelet video encoder SO EURASIP JOURNAL ON ADVANCES IN SIGNAL PROCESSING LA English DT Article DE 3D-DWT; Video coding; GPU; Manycore ID HIERARCHICAL TREES; COEFFICIENTS; COMPRESSION; SPIHT AB The 3D-DWT is a mathematical tool of increasing importance in those applications that require an efficient processing of huge amounts of volumetric info. Other applications like professional video editing, video surveillance applications, multi-spectral satellite imaging, HQ video delivery, etc, would rather use 3D-DWT encoders to reconstruct a frame as fast as possible. In this article, we introduce a fast GPU-based encoder which uses 3D-DWT transform and lower trees. Also, we present an exhaustive analysis of the use of GPU memory. Our proposal shows good trade off between R/D, coding delay (as fast as MPEG-2 for High definition) and memory requirements (up to 6 times less memory than x264). C1 [Galiano, Vicente; Lopez-Granado, Otoniel; Malumbres, Manuel P.; Migallon, Hector] Miguel Hernandez Univ, Phys & Comp Architecture Dept, Elche 03202, Spain. [Drummond, Leroy Anthony] Lawrence Berkeley Natl Lab, Berkeley, CA 94703 USA. RP Galiano, V (reprint author), Miguel Hernandez Univ, Phys & Comp Architecture Dept, Elche 03202, Spain. EM vgaliano@umh.es RI Migallon, Hector/E-3700-2015 OI Migallon, Hector/0000-0002-4937-0905 FU Spanish Ministry of Education and Science [TIN2011-27543-C03-03]; Spanish Ministry of Science and Innovation [TIN2011-26254, TEC2010-11776-E] FX This research was supported by the Spanish Ministry of Education and Science under grant TIN2011-27543-C03-03 and the Spanish Ministry of Science and Innovation under grant number TIN2011-26254 and TEC2010-11776-E. NR 18 TC 1 Z9 1 U1 0 U2 3 PU SPRINGER INTERNATIONAL PUBLISHING AG PI CHAM PA GEWERBESTRASSE 11, CHAM, CH-6330, SWITZERLAND SN 1687-6180 J9 EURASIP J ADV SIG PR JI EURASIP J. Adv. Signal Process. PY 2013 AR 24 DI 10.1186/1687-6180-2013-24 PG 13 WC Engineering, Electrical & Electronic SC Engineering GA 110SW UT WOS:000316467100001 ER PT J AU Richter, S Kuhn, H Truyens, J Kraiem, M Aregbe, Y AF Richter, S. Kuhn, H. Truyens, J. Kraiem, M. Aregbe, Y. TI Uranium hexafluoride (UF6) gas source mass spectrometry for certification of reference materials and nuclear safeguard measurements at IRMM SO JOURNAL OF ANALYTICAL ATOMIC SPECTROMETRY LA English DT Article ID ISOTOPE RATIO MEASUREMENTS AB Uranium hexafluoride gas source mass spectrometry at IRMM is based on two foundations, firstly the operation of a UF6 gas source mass spectrometer (GSMS) and secondly the preparation of primary UF6 reference materials, which were converted from gravimetrically prepared mixtures of highly enriched oxides of U-235 and U-238. Recently a new GSMS for uranium isotopic measurements using UF6 gas, the "URANUS" from Thermo Fisher, was installed at IRMM, which also allows measurements of the so-called "minor" isotope ratios n(U-234)/n(U-238) and n(U-236)/n(U-238). In this paper the design and the implementation of measurement techniques for the new URANUS GSMS are described. This includes the "single standard" and the "double standard" (DS) method as well as the newly developed "memory corrected double standard" method (MCDS). This required a detailed investigation of memory effects within the GSMS instrument, in particular regarding the dependence of memory effects on the isotope ratios of samples and standards. The results of this study led to new recommendations for the selection of the standards for a given sample and for suitable measurement procedures. The measurement performance for the "major" isotope ratio n(U-235)/n(U-238) as well as the "minor" isotope ratios n(U-234)/n(U-238) and n(U-236)/n(U-238) is presented and compared with other mass spectrometric techniques. With the installation and validation of the new URANUS GSMS instrument IRMM has established two new complementary techniques for measuring the full isotopic composition of uranium samples. UF6 GSMS in combination with the MCDS method is considered the preferred technique for samples in the UF6 form and for smaller uncertainties for measurements of the major ratio n(U-235)/n(U-238), while thermal ionization mass spectrometry (TIMS), in combination with the "modified total evaporation" (MTE) method as well as ion counting and high abundance sensitivity for the detection of U-236, provides a superior measurement performance for the minor isotope ratios n(U-234)/n(U-238) and n(U-236)/n(U-238). C1 [Richter, S.; Kuhn, H.; Truyens, J.; Aregbe, Y.] Commiss European Communities, Joint Res Ctr, IRMM, B-2440 Geel, Belgium. [Kraiem, M.] US DOE, NBL, Argonne, IL 60439 USA. RP Richter, S (reprint author), Commiss European Communities, Joint Res Ctr, IRMM, Retieseweg 111, B-2440 Geel, Belgium. EM stephan.richter@ec.europa.eu NR 10 TC 5 Z9 5 U1 1 U2 13 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 0267-9477 J9 J ANAL ATOM SPECTROM JI J. Anal. At. Spectrom. PY 2013 VL 28 IS 4 BP 536 EP 548 DI 10.1039/c3ja30364k PG 13 WC Chemistry, Analytical; Spectroscopy SC Chemistry; Spectroscopy GA 106CD UT WOS:000316118100013 ER PT J AU Zhang, S Shao, YY Yin, GP Lin, YH AF Zhang, Sheng Shao, Yuyan Yin, Geping Lin, Yuehe TI Recent progress in nanostructured electrocatalysts for PEM fuel cells SO JOURNAL OF MATERIALS CHEMISTRY A LA English DT Article ID OXYGEN-REDUCTION REACTION; METAL-FREE ELECTROCATALYSTS; FUNCTIONALIZED GRAPHENE SHEETS; GRAPHITIC MESOPOROUS CARBON; OXIDE-SUPPORTED PLATINUM; CATALYST-FREE SYNTHESIS; FORMIC-ACID OXIDATION; METHANOL OXIDATION; STABLE ELECTROCATALYSTS; ALLOY NANOPARTICLES AB Polymer electrolyte membrane (PEM) fuel cells are attracting much attention as promising clean power sources and an alternative to conventional internal combustion engines, secondary batteries, and other power sources. Much effort from government laboratories, industry, and academia has been devoted to developing PEM fuel cells, and great advances have been achieved. Although prototype cars powered by fuel cells have been delivered, successful commercialization requires fuel cell electrocatalysts, which are crucial components at the heart of fuel cells, meet exacting performance targets. In this review, we present a brief overview of the recent progress in fuel cell electrocatalysts, which involves catalyst supports, Pt and Pt-based electrocatalysts, and non-Pt electrocatalysts. C1 [Zhang, Sheng; Yin, Geping] Harbin Inst Technol, Sch Chem Engn & Technol, Harbin 150001, Peoples R China. [Shao, Yuyan; Lin, Yuehe] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Zhang, S (reprint author), Harbin Inst Technol, Sch Chem Engn & Technol, Harbin 150001, Peoples R China. EM zhangsheng1982@hit.edu.cn; yuehe.lin@pnl.gov RI Zhang, Sheng/H-2452-2011; Shao, Yuyan/A-9911-2008; Lin, Yuehe/D-9762-2011 OI Zhang, Sheng/0000-0001-7532-1923; Shao, Yuyan/0000-0001-5735-2670; Lin, Yuehe/0000-0003-3791-7587 FU National Natural Science Foundation of China [21106024, 21173062]; US-DOE [DE-AC05-76RL01830] FX This work is supported by National Natural Science Foundation of China (Grant nos 21106024 and 21173062). Pacific Northwest National Laboratory is operated by Battelle for US-DOE under Contract DE-AC05-76RL01830. NR 137 TC 87 Z9 88 U1 17 U2 214 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2050-7488 J9 J MATER CHEM A JI J. Mater. Chem. A PY 2013 VL 1 IS 15 BP 4631 EP 4641 DI 10.1039/c3ta01161e PG 11 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Energy & Fuels; Materials Science GA 108HI UT WOS:000316282800002 ER PT J AU Acharya, S Alvarado, J Banerjee, D Billups, WE Chen, G Cola, BA Cross, W Duke, E Graham, S He, H Hong, H Jin, S Karna, S Li, C Li, CH Li, J Peterson, GP Puszynski, JA Routbort, J Shan, J Shin, D Smirnova, A Smith, P Wang, X Waynick, A White, R Yan, X Yu, W AF Acharya, S. Alvarado, J. Banerjee, D. Billups, W. E. Chen, G. Cola, B. A. Cross, W. Duke, E. Graham, S., Jr. He, H. Hong, H. Jin, S. Karna, S. Li, C. Li, C. H. Li, J. Peterson, G. P. Puszynski, J. A. Routbort, J. Shan, J. Shin, D. Smirnova, A. Smith, P. Wang, X. Waynick, A. White, R. Yan, X. Yu, W. TI Report on Carbon Nano Material Workshop: Challenges and Opportunities SO NANOSCALE AND MICROSCALE THERMOPHYSICAL ENGINEERING LA English DT Article DE carbon nanomaterial; thermal property; nanofluids; carbon nanotube; graphene AB The objective of this workshop was to focus on new directions in carbon nanomaterial research, with a particular focus on new frontiers in nanotube alignment and applications of nanofluids. The first Carbon Nano Material Workshop was held at the Radisson Hotel, Rapid City, South Dakota, from October 30 to November 1, 2011, and was organized by Dr. G. P. Bud Peterson, Georgia Institute of Technology, and Dr. Haiping Hong, South Dakota School of Mines and Technology. More than 70 people from various government agencies, national labs, universities, and industries attended the workshop. The workshop agenda follows. The workshop included keynote plenary sessions and invited and contributed sessions, as well as a dedicated poster session of selected presentations assembled from an open call for papers. C1 [Acharya, S.] Natl Sci Fdn, Arlington, VA USA. [Alvarado, J.; Banerjee, D.] Texas A&M Univ, Dept Mech Engn, College Stn, TX 77843 USA. [Billups, W. E.] Rice Univ, Dept Chem, Houston, TX USA. [Chen, G.] MIT, Dept Mech Engn, Cambridge, MA 02139 USA. [Cola, B. A.; Graham, S., Jr.; Peterson, G. P.] Georgia Inst Technol, George W Woodruff Sch Mech Engn, Atlanta, GA 30332 USA. [Cross, W.; Hong, H.] South Dakota Sch Mines & Technol, Dept Mat & Met Engn, Rapid City, SD 57701 USA. [Duke, E.] South Dakota Sch Mines & Technol, South Dakota NASA EPSCoR, Rapid City, SD 57701 USA. [He, H.] Rutgers State Univ, Dept Chem, Newark, NJ 07102 USA. [Jin, S.] Univ Calif San Diego, Dept Mech & Aerosp Engn, San Diego, CA 92103 USA. [Karna, S.; Smith, P.] USA, Res Lab, Aberdeen Proving Ground, MD USA. [Li, C.] Univ S Carolina, Dept Mech Engn, Columbia, SC 29208 USA. [Li, C. H.] Villanova Univ, Dept Mech Engn, Villanova, PA 19085 USA. [Li, J.] NASA, Ctr Nanotechnol, Ames Res Lab, Moffett Field, CA USA. [Puszynski, J. A.] South Dakota Sch Mines & Technol, Dept Chem & Biol Engn, Rapid City, SD 57701 USA. [Routbort, J.; Yu, W.] Argonne Natl Lab, Div Energy Syst, Argonne, IL 60439 USA. [Shan, J.] Rutgers State Univ, Dept Mech & Aerosp Engn, Piscataway, NJ 08855 USA. [Shin, D.] Univ Texas Arlington, Dept Mech & Aerosp Engn, Arlington, TX 76019 USA. [Smirnova, A.] South Dakota Sch Mines & Technol, Dept Chem, Rapid City, SD 57701 USA. [Wang, X.] Iowa State Univ, Dept Mech Engn, Ames, IA USA. [Waynick, A.] NCH Corp, R&D Div, Irving, TX USA. [White, R.] South Dakota Sch Mines & Technol, Off Res, Rapid City, SD 57701 USA. [Yan, X.] S Dakota State Univ, Dept Elect Engn & Comp Sci, Brookings, SD 57007 USA. RP Hong, H (reprint author), South Dakota Sch Mines & Technol, Dept Mat & Met Engn, 501 St Joseph St, Rapid City, SD 57701 USA. EM Haiping.Hong@sdsmt.edu RI Cola, Baratunde/N-1903-2013; YAN, Xingzhong/B-5074-2011; Chen, Gang/J-1325-2014; Li, Calvin Hong/B-6905-2009; OI Cola, Baratunde/0000-0003-1268-9573; Chen, Gang/0000-0002-3968-8530; Alvarado, Jorge/0000-0002-4059-6588 FU South Dakota School of Mines and Technology; Georgia Institute of Technology; U.S. Army Research Laboratory; South Dakota NASA Experimental Program to Stimulate Competitive Research (EPSCoR); National Science Foundation FX This workshop was financially supported by the South Dakota School of Mines and Technology, the Georgia Institute of Technology, the U.S. Army Research Laboratory, the South Dakota NASA Experimental Program to Stimulate Competitive Research (EPSCoR), and the National Science Foundation. NR 28 TC 3 Z9 3 U1 0 U2 16 PU TAYLOR & FRANCIS INC PI PHILADELPHIA PA 530 WALNUT STREET, STE 850, PHILADELPHIA, PA 19106 USA SN 1556-7265 EI 1556-7273 J9 NANOSC MICROSC THERM JI Nanoscale Microscale Thermophys. Eng. PD JAN 1 PY 2013 VL 17 IS 1 BP 10 EP 24 DI 10.1080/15567265.2012.745912 PG 15 WC Thermodynamics; Engineering, Mechanical; Nanoscience & Nanotechnology; Materials Science, Characterization & Testing; Physics, Applied SC Thermodynamics; Engineering; Science & Technology - Other Topics; Materials Science; Physics GA 105IA UT WOS:000316059000002 ER PT J AU Gongora-Castillo, E Buell, CR AF Gongora-Castillo, Elsa Buell, C. Robin TI Bioinformatics challenges in de novo transcriptome assembly using short read sequences in the absence of a reference genome sequence SO NATURAL PRODUCT REPORTS LA English DT Review ID RNA-SEQ; LEAF TRANSCRIPTOME; GENE-EXPRESSION; BIOSYNTHESIS; REVEALS; ANNOTATION; PATTERNS; DISCOVERY; DYNAMICS; PROTEIN AB Plant natural product research can be facilitated through genome and transcriptome sequencing approaches that generate informative sequence and expression datasets that enable characterization of biochemical pathways of interest. As the overwhelming majority of plant-derived natural products are derived from species with little, if any, sequence and/or genomic resources, the ability to perform whole genome shotgun sequencing and assembly has been and will continue to be transformative as access to a genome sequence provides molecular resources and a context for discovery and characterization of biosynthetic pathways. Due to the reduced size and complexity of the transcriptome relative to the genome, transcriptome sequencing provides a rapid, inexpensive approach to access gene sequences, gene expression abundances, and gene expression patterns in any species, including those that lack a reference genome sequence. To date, successful applications of RNA sequencing in conjunction with de novo transcriptome assembly has enabled identification of new genes in an array of biochemical pathways in plants. While sequencing technologies are well developed, challenges remain in the handling and analysis of transcriptome sequences. In this Highlight article, we provide an overview of the bioinformatics challenges associated with transcriptome analyses using short read sequences and how to address these issues in plant species that lack a reference genome. C1 [Buell, C. Robin] Michigan State Univ, Dept Plant Biol, E Lansing, MI 48824 USA. Michigan State Univ, Dept Energy, Great Lakes Bioenergy Res Ctr, Dept Plant Biol, E Lansing, MI 48824 USA. RP Buell, CR (reprint author), Michigan State Univ, Dept Plant Biol, E Lansing, MI 48824 USA. EM buell@msu.edu RI Gongora, Elsa/R-8854-2016 OI Gongora, Elsa/0000-0001-6327-6993 FU National Institute of General Medical Sciences [1RC2GM092521]; U.S. Department of Agriculture [2009-6530005784, 2009-85606-05673]; U.S. Department of Energy Great Lakes Bioenergy Research Center (DOE BER Office of Science) [DE-FC02-07ER64494]; U.S. National Science Foundation [IOS-0922493, MCB-1121650, DBI-0604907/DBI-0834044] FX Funding for plant transcriptome work was provided by grants to C.R.B. from the National Institute of General Medical Sciences (1RC2GM092521), U.S. Department of Agriculture (2009-6530005784, 2009-85606-05673), U.S. Department of Energy Great Lakes Bioenergy Research Center (DOE BER Office of Science DE-FC02-07ER64494), and U.S. National Science Foundation (IOS-0922493, MCB-1121650, DBI-0604907/DBI-0834044). The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 61 TC 21 Z9 22 U1 5 U2 109 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 0265-0568 J9 NAT PROD REP JI Nat. Prod. Rep. PY 2013 VL 30 IS 4 BP 490 EP 500 DI 10.1039/c3np20099j PG 11 WC Biochemistry & Molecular Biology; Chemistry, Medicinal; Chemistry, Organic SC Biochemistry & Molecular Biology; Pharmacology & Pharmacy; Chemistry GA 104BK UT WOS:000315964000002 PM 23377493 ER PT J AU McMahon, JM Schatz, GC Gray, SK AF McMahon, Jeffrey M. Schatz, George C. Gray, Stephen K. TI Plasmonics in the ultraviolet with the poor metals Al, Ga, In, Sn, Tl, Pb, and Bi SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID SURFACE-ENHANCED SPECTROSCOPY; OPTICAL-PROPERTIES; ALUMINUM NANOPARTICLES; RESONANCE SPECTROSCOPY; GALLIUM NANOPARTICLES; RAMAN-SCATTERING; FILMS; FLUORESCENCE; ABSORPTION; THALLIUM AB We discuss how the poor metals Al, Ga, In, Sn, Tl, Pb, and Bi can be used for plasmonics in the near to far ultraviolet (UV) range, similar to the noble metals Ag and Au in the visible (Vis) range. We first discuss the empirical dielectric functions of the poor metals, contrasting them with Ag and Au, and also fitting them to a Drude and multiple Lorentz oscillator form. Using Mie theory, we then compare the optical responses of spherical poor metal nanoparticles to noble metal ones. Finally, nanoparticle dimers are studied using a vectorial finite element method. We show how the poor metals exhibit large electric field enhancements in the UV, comparable to Au in the Vis, which makes them particularly attractive for sensing applications, such as surface enhanced Raman spectroscopy. C1 [McMahon, Jeffrey M.; Schatz, George C.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [McMahon, Jeffrey M.; Gray, Stephen K.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. RP Gray, SK (reprint author), Argonne Natl Lab, Ctr Nanoscale Mat, 9700 S Cass Ave, Argonne, IL 60439 USA. EM gray@anl.gov FU NSF MRSEC at the Materials Research Center of Northwestern University [DMR-1121262]; Center for Nanoscale Materials, a U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility [DE-AC02-06CH11357] FX J.M.M. and G. C. S. were supported by the NSF MRSEC (DMR-1121262) at the Materials Research Center of Northwestern University. This work was performed, in part, at the Center for Nanoscale Materials, a U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility under Contract No. DE-AC02-06CH11357. NR 38 TC 85 Z9 85 U1 9 U2 126 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PY 2013 VL 15 IS 15 BP 5415 EP 5423 DI 10.1039/c3cp43856b PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 110TD UT WOS:000316467800017 PM 23429382 ER PT J AU Kobayashi, T Lafon, O Thankamony, ASL Slowing, II Kandel, K Carnevale, D Vitzthum, V Vezin, H Amoureux, JP Bodenhausen, G Pruski, M AF Kobayashi, Takeshi Lafon, Olivier Thankamony, Aany S. Lilly Slowing, Igor I. Kandel, Kapil Carnevale, Diego Vitzthum, Veronika Vezin, Herve Amoureux, Jean-Paul Bodenhausen, Geoffrey Pruski, Marek TI Analysis of sensitivity enhancement by dynamic nuclear polarization in solid-state NMR: a case study of functionalized mesoporous materials SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID THEORETICAL CALCULATIONS; SILICA NANOPARTICLES; ROTATING SOLIDS; LOW-TEMPERATURE; CHEMICAL-SHIFT; SI-29 NMR; MAS-NMR; SPECTROSCOPY; PROTEINS; RELAXATION AB We systematically studied the enhancement factor (per scan) and the sensitivity enhancement (per unit time) in C-13 and Si-29 cross-polarization magic angle spinning (CP-MAS) NMR boosted by dynamic nuclear polarization (DNP) of functionalized mesoporous silica nanoparticles (MSNs). Specifically, we separated contributions due to: (i) microwave irradiation, (ii) quenching by paramagnetic effects, (iii) the presence of frozen solvent, (iv) the temperature, as well as changes in (v) relaxation and (vi) cross-polarization behaviour. No line-broadening effects were observed for MSNs when lowering the temperature from 300 to 100 K. Notwithstanding a significant signal reduction due to quenching by TOTAPOL radicals, DNP-CP-MAS at 100 K provided global sensitivity enhancements of 23 and 45 for C-13 and Si-29, respectively, relative to standard CP-MAS measurements at room temperature. The effects of DNP were also ascertained by comparing with state-of-the-art two-dimensional heteronuclear H-1{C-13} and Si-29{H-1} correlation spectra, using, respectively, indirect detection or Carr-Purcell-Meiboom-Gill (CPMG) refocusing to boost signal acquisition. This study highlights opportunities for further improvements through the development of high-field DNP, better polarizing agents, and improved capabilities for low-temperature MAS. C1 [Kobayashi, Takeshi; Slowing, Igor I.; Kandel, Kapil; Pruski, Marek] US DOE, Ames Lab, Ames, IA 50011 USA. [Lafon, Olivier; Thankamony, Aany S. Lilly; Vezin, Herve; Amoureux, Jean-Paul] Univ Lille Nord de France, F-59000 Lille, France. [Lafon, Olivier; Thankamony, Aany S. Lilly; Amoureux, Jean-Paul] Univ Lille 1, Ecole Natl Super Chim Lille, CNRS, Unite Catalyse & Chim Solide,UMR 8181, F-59652 Villeneuve Dascq, France. [Carnevale, Diego; Vitzthum, Veronika; Bodenhausen, Geoffrey] Ecole Polytech Fed Lausanne, EPFL, Inst Sci & Ingn Chim, CH-1015 Lausanne, Switzerland. [Vezin, Herve] Univ Lille 1, Lab Spectrochim Infrarouge & Raman LASIR, CNRS, UMR 8516, F-59652 Villeneuve Dascq, France. [Bodenhausen, Geoffrey] Univ Paris 06, CNRS, UMR 7203, Ecole Normale Super,Dept Chim, Paris, France. [Kandel, Kapil; Pruski, Marek] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. RP Pruski, M (reprint author), US DOE, Ames Lab, Ames, IA 50011 USA. EM mpruski@iastate.edu RI Vezin, Herve/I-8004-2015; Lafon, Olivier/H-1046-2012; OI Vezin, Herve/0000-0002-7282-2703; Lafon, Olivier/0000-0002-5214-4060; Slowing, Igor/0000-0002-9319-8639 FU Ames Laboratory by the U.S. Department of Energy, Office of Basic Energy Sciences; U.S. Department of Energy by Iowa State University [DE-AC02-07CH11358]; Region Nord/Pas de Calais, Europe (FEDER); CNRS; French Ministry of Science [FR-3050]; USTL; ENSCL; Bruker BioSpin; MPNS COST Action EUROHyperPOL [TD1103]; ANR [2010-JCJC-0811-01]; Commission for Technology and Innovation (CTI); Swiss National Science Foundation (SNSF); EPFL FX This research was supported at the Ames Laboratory by the U.S. Department of Energy, Office of Basic Energy Sciences. Ames Laboratory is operated for the U.S. Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. In Lille, this research was supported by the Region Nord/Pas de Calais, Europe (FEDER), the CNRS, the French Ministry of Science, FR-3050, USTL, ENSCL, Bruker BioSpin, MPNS COST Action EUROHyperPOL TD1103, and the ANR under contract 2010-JCJC-0811-01. In Lausanne, this work was supported by the Commission for Technology and Innovation (CTI), the Swiss National Science Foundation (SNSF) and the EPFL. NR 60 TC 33 Z9 33 U1 4 U2 101 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PY 2013 VL 15 IS 15 BP 5553 EP 5562 DI 10.1039/c3cp00039g PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 110TD UT WOS:000316467800031 PM 23459985 ER PT J AU Du, P Lu, J Lau, KC Luo, XY Bareno, J Zhang, XY Ren, Y Zhang, ZC Curtiss, LA Sun, YK Amine, K AF Du, Peng Lu, Jun Lau, Kah Chun Luo, Xiangyi Bareno, Javier Zhang, Xiaoyi Ren, Yang Zhang, Zhengcheng Curtiss, Larry A. Sun, Yang-Kook Amine, Khalil TI Compatibility of lithium salts with solvent of the non-aqueous electrolyte in Li-O-2 batteries SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID LI-AIR BATTERIES; CARBONATE ELECTROLYTES; POLYMER ELECTROLYTE; ELECTROCHEMISTRY; CHALLENGES; NANOWIRES; STABILITY; CHEMISTRY AB The stability of lithium salts, especially in the presence of reduced oxygen species, O-2 and H2O (even in a small amount), plays an important role in the cyclability and capacity of Li-O-2 cells. This combined experimental and computational study provides evidence that the stability of the electrolyte used in Li-O-2 cells strongly depends on the compatibility of lithium salts with solvent. In the case of the LiPF6-1NM(3) electrolyte, the decomposition of LiPF6 occurs in the cell as evidenced by in situ XRD, FT-IR and XPS analysis, which triggers the decomposition of 1NM3 solvent due to formation of HF from the decomposition of LiPF6. These reactions lead to degradation of the electrolyte and cause poor cyclability of the cell. The same reactions are not observed when LiTFSI and LiCF3SO3 are used as the lithium salts in 1NM3 solvent, or LiPF6 is used in TEGDME solvent. C1 [Du, Peng; Lu, Jun; Luo, Xiangyi; Bareno, Javier; Zhang, Zhengcheng; Amine, Khalil] Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA. [Lau, Kah Chun; Curtiss, Larry A.] Argonne Natl Lab, Div Mat Sci, Lemont, IL 60439 USA. [Luo, Xiangyi] Univ Utah, Dept Met Engn, Salt Lake City, UT 84112 USA. [Zhang, Xiaoyi; Ren, Yang] Argonne Natl Lab, Xray Sci Div, Adv Photon Source, Lemont, IL 60439 USA. [Sun, Yang-Kook] Hanyang Univ, Dept WCU Energy Engn, Seoul 133791, South Korea. [Sun, Yang-Kook] Hanyang Univ, Dept Chem Engn, Seoul 133791, South Korea. RP Zhang, ZC (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Lemont, IL 60439 USA. EM zzhang@anl.gov; curtiss@anl.gov; amine@anl.gov RI Lau, Kah Chun/A-9348-2013; Du, Peng/F-8336-2013; Amine, Khalil/K-9344-2013; Luo, Xiangyi/N-4709-2014; OI Lau, Kah Chun/0000-0002-4925-3397; Luo, Xiangyi/0000-0002-4817-1461; Bareno, Javier/0000-0003-1230-9278 FU U.S. Department of Energy; U.S. Department of Energy, FreedomCAR and Vehicle Technologies Office; Department of Energy (DOE), Office of Energy Efficiency and Renewable Energy (EERE); DOE [DE-AC05-06OR23100]; Center for Electrical Energy Storage: Tailored Interfaces, an Energy Frontier Research Center; U.S. Department of Energy, Office of Science, and Office of Basic Energy Sciences; Human Resources Development of the Korea Institute of Energy Technology Evaluation and Planning (KETEP); Korean government, Ministry of Knowledge and Economy [20114010203150]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX Research at Argonne National Laboratory was funded by the U.S. Department of Energy, FreedomCAR and Vehicle Technologies Office. J. Lu was supported by the Department of Energy (DOE), Office of Energy Efficiency and Renewable Energy (EERE), Postdoctoral Research Award under the EERE Vehicles Technology Program administered by the Oak Ridge Institute for Science and Education (ORISE) for the DOE. ORISE is managed by Oak Ridge Associated Universities (ORAU) under DOE contract number DE-AC05-06OR23100. Computational studies supported by the Center for Electrical Energy Storage: Tailored Interfaces, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, and Office of Basic Energy Sciences. This work was also supported by the Human Resources Development of the Korea Institute of Energy Technology Evaluation and Planning (KETEP) grant funded by the Korean government, Ministry of Knowledge and Economy (No. 20114010203150). We acknowledge grants of computer time through INCITE and ALCC awards for BlueGene/P computer at Argonne National Laboratory and allocations on the CNM Carbon Cluster at Argonne National Laboratory, the ALCF Fusion Cluster at Argonne National Laboratory, and the EMSL Chinook Cluster at Pacific Northwest National Laboratory. Use of the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under contract no. DE-AC02-06CH11357. NR 41 TC 41 Z9 42 U1 6 U2 152 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PY 2013 VL 15 IS 15 BP 5572 EP 5581 DI 10.1039/c3cp50500f PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 110TD UT WOS:000316467800033 PM 23463031 ER PT J AU Zhang, X Eyles, CJ Taatjes, CA Ding, DJ Stolte, S AF Zhang, Xia Eyles, Chris J. Taatjes, Craig A. Ding, Dajun Stolte, Steven TI A general scaling rule for the collision energy dependence of a rotationally inelastic differential cross-section and its application to NO(X) plus He SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID FINE-STRUCTURE TRANSITIONS; STERIC ASYMMETRY; MOLECULAR-COLLISIONS; QUANTUM TREATMENT; SCATTERING; STATE; AR; VELOCITY; NO; PROPENSITIES AB The quasi-quantum treatment (QQT) (Gijsbertsen et al., J. Am. Chem. Soc., 2006, 128, 8777) provides a physically compelling framework for the evaluation of rotationally inelastic scattering, including the differential cross sections (DCS). In this work the QQT framework is extended to treat the DCS in the classically forbidden region as well as the classically allowed region. Most importantly, the QQT is applied to the collision energy dependence of the angular distributions of these DCSs. This leads to an analytical formalism that reveals a scaling relationship between the DCS calculated at a particular collision energy and the DCS at other collision energies. This scaling is shown to be exact for QM calculated or experimental DCSs if the magnitude of the (kinematic apse frame) underlying scattering amplitude depends solely on the projection of the incoming momentum vector onto the kinematic apse vector. The QM DCSs of the NO(X)-He collision system were found to obey this scaling law nearly perfectly for energies above 63 meV. The mathematical derivation is accompanied by a mechanistic description of the Feynman paths that contribute to the scattering amplitude in the classically allowed and forbidden regions, and the nature of the momentum transfer during the collision process. This scaling relationship highlights the nature of (and limits to) the information that is obtainable from the collision-energy dependence of the DCS, and allows a description of the relevant angular range of the DCSs that embodies this information. C1 [Zhang, Xia; Ding, Dajun; Stolte, Steven] Jilin Univ, Inst Atom & Mol Phys, Changchun 130012, Peoples R China. [Eyles, Chris J.] Max Planck Gesell, Fritz Haber Inst, D-14195 Berlin, Germany. [Taatjes, Craig A.] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA. [Stolte, Steven] Vrije Univ, Fac Exact Sci, Ctr Laser, NL-1081 HV Amsterdam, Netherlands. [Stolte, Steven] CEA Saclay, Lab Francis Perrin, DRECEM, SPAM, F-91191 Gif Sur Yvette, France. RP Ding, DJ (reprint author), Jilin Univ, Inst Atom & Mol Phys, Changchun 130012, Peoples R China. EM dajund@jlu.edu.cn; s.stolte@vu.nl FU National Natural Science Foundation of China [11034003, 91221301]; National Basic Research Program of China [2013CB922200]; Division of Chemical Sciences, Geosciences, and Biosciences, in the Office of Basic Energy Sciences of the United States Department of Energy; National Nuclear Security Administration [DE-AC04-94-AL85000] FX We are grateful to Dr J. Klos for making available the complete set of He-NO(X) HIBRIDON QM DCS tables at EcolH = 147 meV and EcolL = 63 meV. This work is supported by the National Natural Science Foundation of China under grants no. 11034003 and 91221301, the National Basic Research Program of China under grant no. 2013CB922200. C.A.T. is supported by the Division of Chemical Sciences, Geosciences, and Biosciences, in the Office of Basic Energy Sciences of the United States Department of Energy. Sandia is a multi-program laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the National Nuclear Security Administration under contract DE-AC04-94-AL85000. NR 46 TC 2 Z9 2 U1 0 U2 16 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PY 2013 VL 15 IS 15 BP 5620 EP 5635 DI 10.1039/c3cp50558h PG 16 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 110TD UT WOS:000316467800037 PM 23471220 ER PT J AU Laissue, JA Bartzsch, S Blattmann, H Brauer-Krisch, E Bravin, A Dallery, D Djonov, V Hanson, AL Hopewell, JW Kaser-Hotz, B Keyrilainen, J Laissue, PP Miura, M Serduc, R Siegbahn, AE Slatkin, DN AF Laissue, Jean A. Bartzsch, Stefan Blattmann, Hans Braeuer-Krisch, Elke Bravin, Alberto Dallery, Dominique Djonov, Valentin Hanson, Albert L. Hopewell, John W. Kaser-Hotz, Barbara Keyrilainen, Jani Laissue, Pierre Philippe Miura, Michiko Serduc, Raphael Siegbahn, Albert E. Slatkin, Daniel N. TI Response of the rat spinal cord to X-ray microbeams SO RADIOTHERAPY AND ONCOLOGY LA English DT Article DE Spinal cord response; Synchrotron X-rays; Microbeams ID CENTRAL-NERVOUS-SYSTEM; RADIATION-THERAPY; IRRADIATION; BRAIN; TOLERANCE; BEAMS; RADIOTHERAPY; REPAIR; MOUSE AB Background and purpose: To quantify the late,close-related responses of the rat cervical spinal cord to Xray irradiations by an array of microbeams or by a single millimeter beam. Materials and methods: Necks of anesthetized rats were irradiated transversely by an 11 mm wide array of 52 parallel, 35 gm wide, vertical X-ray microbeams, separated by 210 mu m intervals between centers. Comparison was made with rats irradiated with a 1.35 mm wide single beam of similar X-rays. Rats were killed when paresis developed, or up to 383 days post irradiation (dpi). Results: Microbeam peak/valley doses of approximate to 1357/12.7 Gy to 715/25.4 Gy to an 11 mm long segment of the spinal cord, or single beam doses of approximate to 146-454 Gy to a 1.35 mm long segment caused foreleg paresis and histopathologically verified spinal cord damage; rats exposed to peak/valley doses up to 253/9 Gy were paresis-free at 383 dpi. Conclusions: Whereas microbeam radiation therapy [MRT] for malignant gliomas implanted in rat brains can be safe, palliative or curative, the high tolerance of normal rat spinal cords to similar microbeam exposures justifies testing MRT for autochthonous malignancies in the central nervous system of larger animals with a view to subsequent clinical applications. (C) 2012 Elsevier Ireland Ltd. All rights reserved. Radiotherapy and Oncology 106 (2013) 106-111 C1 [Laissue, Jean A.; Blattmann, Hans] Univ Bern, Inst Pathol, CH-3012 Bern, Switzerland. [Bartzsch, Stefan] Deutsch Krebsforschungszentrum, Heidelberg, Germany. [Braeuer-Krisch, Elke; Bravin, Alberto; Dallery, Dominique] European Synchrotron Radiat Facil, F-38043 Grenoble, France. [Djonov, Valentin] Univ Bern, Inst Anat, Bern, Switzerland. [Hanson, Albert L.; Miura, Michiko] Brookhaven Natl Lab, Upton, NY 11973 USA. [Hopewell, John W.] Univ Oxford, Particle Therapy Canc Res Inst, Oxford OX1 2JD, England. [Kaser-Hotz, Barbara] Anim Oncol & Imaging Ctr, Hunenberg, Switzerland. [Keyrilainen, Jani] Univ Helsinki, Cent Hosp, Dept Phys, FIN-00014 Helsinki, Finland. [Laissue, Pierre Philippe] Univ Essex, Dept Biol Sci, Colchester CO4 3SQ, Essex, England. [Serduc, Raphael] INSERM, U836, Grenoble, France. [Serduc, Raphael] Univ Grenoble 1, Grenoble Inst Neurosci, Grenoble, France. [Siegbahn, Albert E.] Karolinska Univ Hosp, Dept Med Phys, Stockholm, Sweden. [Slatkin, Daniel N.] Nanoprobes Inc, Yaphank, NY USA. RP Laissue, JA (reprint author), Aarwylweg 7, CH-3074 Muri Bern, Switzerland. EM laissue@pathology.unibe.ch RI Bravin, Alberto/R-8633-2016; OI Bravin, Alberto/0000-0001-6868-2755; Siegbahn, Albert/0000-0002-1491-487X FU Institute of Pathology, University of Bern, Switzerland; ESRF; Microbeam Therapy, LLC (San Carlos, CA USA) FX This research was funded by the Institute of Pathology, University of Bern, Switzerland, and by the ESRF. We also thank Microbeam Therapy, LLC (San Carlos, CA USA), for supporting MM and DNS. NR 31 TC 13 Z9 13 U1 0 U2 16 PU ELSEVIER IRELAND LTD PI CLARE PA ELSEVIER HOUSE, BROOKVALE PLAZA, EAST PARK SHANNON, CO, CLARE, 00000, IRELAND SN 0167-8140 J9 RADIOTHER ONCOL JI Radiother. Oncol. PD JAN PY 2013 VL 106 IS 1 BP 106 EP 111 DI 10.1016/j.radonc.2012.12.007 PG 6 WC Oncology; Radiology, Nuclear Medicine & Medical Imaging SC Oncology; Radiology, Nuclear Medicine & Medical Imaging GA 108NY UT WOS:000316303800018 PM 23321495 ER PT J AU Lu, J Pan, YX Wang, JG Chen, X Huang, SM Liu, GK AF Lu, Jing Pan, Yuexiao Wang, Jiaguo Chen, Xi'an Huang, Shaoming Liu, Guokui TI Reduction of Mn4+ to Mn2+ in CaAl12O19 by co-doping charge compensators to obtain tunable photoluminescence SO RSC ADVANCES LA English DT Article ID LUMINESCENCE; PHOSPHOR; FLUORESCENCE; ENHANCEMENT; HIBONITE; EU3+; EU2+ AB Green and red photoluminescence (PL) is obtained from manganese activated phosphor CaAl12O19 (CAO) synthesized using a solid-state reaction method. The red PL is attributed to Mn4+ at an octahedral Al3+ site and the green PL is from Mn2+ at a tetrahedral Al3+ site. Thermal reduction of Mn4+ to Mn2+ in CAO lattice does not complete, even in a reducing atmosphere, but can be fully realized through co-doping of trivalent ions such as Bi3+ and La3+ with ion radii similar to that of Ca2+. The intensity of the Mn2+ green luminescence strongly depends on the co-doping concentration of the trivalent ions. C1 [Lu, Jing; Pan, Yuexiao; Wang, Jiaguo; Chen, Xi'an; Huang, Shaoming] Wenzhou Univ, Fac Chem & Mat Engn, Nanomat & Chem Key Lab, Wenzhou 325027, Zhejiang, Peoples R China. [Liu, Guokui] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Pan, YX (reprint author), Wenzhou Univ, Fac Chem & Mat Engn, Nanomat & Chem Key Lab, Wenzhou 325027, Zhejiang, Peoples R China. EM yxpan8@gmail.com; gkliu@anl.gov FU Zhejiang Provincial NSF [Y4100299]; Chinese National NSF [51102185, 51025207]; U.S. Department of Energy [DE-AC02-06CH11357] FX This research was jointly supported by Zhejiang Provincial NSF (Grant No. Y4100299) and Chinese National NSF (Grant No. 51102185, 51025207). Work performed at Argonne National Laboratory was supported by the U.S. Department of Energy under contract DE-AC02-06CH11357. NR 20 TC 11 Z9 11 U1 2 U2 56 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2046-2069 J9 RSC ADV JI RSC Adv. PY 2013 VL 3 IS 14 BP 4510 EP 4513 DI 10.1039/c3ra22938f PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA 103HC UT WOS:000315905400006 ER PT J AU Yamaguchi, H Gin, P Arita, H Kobayashi, M Bennett, S Satija, SK Asada, M Koga, T Takahara, A AF Yamaguchi, Hiroki Gin, Peter Arita, Hiroshi Kobayashi, Motoyasu Bennett, Steve Satija, Sushil K. Asada, Mitsunori Koga, Tadanori Takahara, Atsushi TI Effect of supercritical carbon dioxide on molecular aggregation states of side chains of semicrystalline poly{2-(perfluorooctyl)ethyl acrylate} brush thin films SO RSC ADVANCES LA English DT Article ID TRANSFER RADICAL POLYMERIZATION; X-RAY-DIFFRACTION; NEUTRON REFLECTIVITY; ELEVATED PRESSURES; SORPTION; FLUIDS; POLYMERS; FLUOROALCOHOL; SOLVENTS; BEHAVIOR AB We report a carbon dioxide-based approach to induce highly ordered molecular aggregation states of perfluoroalkyl (R-f) chains of densely-grafted poly{2-(perfluorooctyl)ethyl acrylate} (poly(FA-C-8)) brush in place of conventional thermal annealing. Poly(FA-C-8) brush films of 40 nm thickness were prepared by surface-initiated atom transfer radical polymerization. In-situ neutron reflectivity measurements for the poly(FA-C-8) brush films under the isothermal condition of T = 309 K, which is below the bulk melting temperature (T-m = 348 K), elucidated large expansion of polymer chains due to sorption of CO2 molecules. Comparison of the swelling behavior with an amorphous poly{2-(perfluorobutyl)ethyl acrylate} brush thin film clarified that the sorption of CO2 molecules results in the melting of the semicrystalline poly(FA-C-8) brush at P > 4.1 MPa. In addition, by using out-of-plane grazing incidence wide-angle X-ray diffraction, it was found that subsequent slow quench from P > 4.1 MPa induces rearrangement of the rigid rod-like R-f groups, forming highly ordered molecular aggregation structures similar to those via a conventional thermal process. The appropriate CO2 process conditions for the effective induction of the highly ordered structures of the rigid R-f groups are discussed in detail. C1 [Yamaguchi, Hiroki; Arita, Hiroshi; Takahara, Atsushi] Kyushu Univ, Grad Sch Engn, Nishi Ku, Fukuoka 8190395, Japan. [Gin, Peter; Asada, Mitsunori; Koga, Tadanori] SUNY Stony Brook, Dept Mat Sci & Engn, Stony Brook, NY 11974 USA. [Kobayashi, Motoyasu] Kyushu Univ, Inst Mat Chem & Engn, Nishi Ku, Fukuoka 8190395, Japan. [Kobayashi, Motoyasu] Japan Sci & Technol Agcy, ERATO Takahara Soft Interfaces Project, Nishi Ku, Fukuoka 8190395, Japan. [Bennett, Steve] Brookhaven Natl Lab, Natl Synchrotron Light Source, Upton, NY 11973 USA. [Satija, Sushil K.] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Asada, Mitsunori; Koga, Tadanori] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11974 USA. [Takahara, Atsushi] Kyushu Univ, Int Inst Carbon Neutral Energy Res WPI I2CNER, Fukuoka 8190395, Japan. RP Yamaguchi, H (reprint author), Kyushu Univ, Grad Sch Engn, Nishi Ku, 744 Motooka, Fukuoka 8190395, Japan. EM tadanori.koga@stonybrook.edu; takahara@cstf.kyushu-u.ac.jp RI Koga, Tadanori/A-4007-2010; U-ID, Kyushu/C-5291-2016 FU Ministry of Education, Culture, Science, Sports and Technology of Japan [19750098]; NSF Grant [CMMI-0846267] FX The present work is supported by a Grant-in-Aid for the Global COE Program, "Science for Future Molecular Systems", and partially supported by a Grant-in Aid for Young Scientist (B) (19750098) from the Ministry of Education, Culture, Science, Sports and Technology of Japan. H. Y. acknowledges the financial support of a Grant-in-Aid for JSPS Fellows. T. K. acknowledges the financial support from NSF Grant No. CMMI-0846267. We gratefully acknowledge Dr M. Morita (Daikin Industries Co., Ltd.) for the donation of FA-C8 monomer. NR 55 TC 3 Z9 3 U1 2 U2 35 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2046-2069 J9 RSC ADV JI RSC Adv. PY 2013 VL 3 IS 14 BP 4778 EP 4785 DI 10.1039/c3ra22692a PG 8 WC Chemistry, Multidisciplinary SC Chemistry GA 103HC UT WOS:000315905400044 ER PT J AU Sathre, R Masanet, E AF Sathre, Roger Masanet, Eric TI Prospective life-cycle modeling of a carbon capture and storage system using metal-organic frameworks for CO2 capture SO RSC ADVANCES LA English DT Article ID POWER-GENERATION; DIOXIDE CAPTURE; UNITED-STATES; ENERGY; EMISSIONS; TRANSPORT; PLANT; GAS AB Metal-organic frameworks (MOFs) are promising new material media for carbon dioxide (CO2) capture. Their tunable adsorption patterns may allow relatively efficient separation of gases, e.g. from power plant exhaust. Here we conduct scenario-based prospective life-cycle system modeling to estimate the potentials and implications of large-scale MOF application for post-combustion carbon capture and storage (CCS), and estimate the source and magnitude of uncertainties. The methodological approach includes parametric system modeling to quantify relations between system components; scenario projections of plausible pathways for system scale-up; proxy data on analogous materials and processes; and uncertainty analysis of parameter significance. We estimate the system-wide material and energy flows and economic costs associated with projected large-scale CCS deployment. We compare the performance of a MOF-based system to currently more mature amine-based capture technology. We discuss balancing two critical factors that determine the success of CO2 capture media: thermodynamic efficiency of the capture/regeneration cycle, and life-cycle embodied energy and cost of the material and its ancillary systems. C1 [Sathre, Roger] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Masanet, Eric] Northwestern Univ, Dept Mech Engn, Evanston, IL 60208 USA. RP Sathre, R (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. RI Masanet, Eric /I-5649-2012 FU US Department of Energy [DE-AC02-05CH11231, DE-AR0000103]; Advanced Research Projects Agency-Energy (ARPA-E) FX This work was conducted at Lawrence Berkeley National Laboratory under the US Department of Energy Contract No. DE-AC02-05CH11231. The work was funded by the Advanced Research Projects Agency-Energy (ARPA-E), US Department of Energy, under Award No. DE-AR0000103. We thank Jennifer Cain, Mikhail Chester, Kenji Sumida, Adam Berger, Abhoyjit Bhown, Berend Smit, and Jeff Long for their invaluable assistance. NR 57 TC 16 Z9 16 U1 1 U2 46 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2046-2069 J9 RSC ADV JI RSC Adv. PY 2013 VL 3 IS 15 BP 4964 EP 4975 DI 10.1039/c3ra40265g PG 12 WC Chemistry, Multidisciplinary SC Chemistry GA 107OC UT WOS:000316226500020 ER PT J AU Brune, PR Knepley, MG Scott, LR AF Brune, Peter R. Knepley, Matthew G. Scott, L. Ridgway TI UNSTRUCTURED GEOMETRIC MULTIGRID IN TWO AND THREE DIMENSIONS ON COMPLEX AND GRADED MESHES SO SIAM JOURNAL ON SCIENTIFIC COMPUTING LA English DT Article DE finite element method; multigrid; interpolation; meshing ID FINITE-ELEMENT EQUATIONS; QUASI-UNIFORM MESHES; STRATEGIES; DELETE AB The use of multigrid and related preconditioners with the finite element method is often limited by the difficulty of applying the algorithm effectively to a problem, especially when the domain has a complex shape or the mesh has adaptive refinement. We introduce a simplification of a general topologically motivated mesh coarsening algorithm for use in creating hierarchies of meshes for geometric unstructured multigrid methods. The connections between the guarantees of this technique and the quality criteria necessary for multigrid methods for nonquasi-uniform problems are noted. The implementation details, in particular those related to coarsening, remeshing, and interpolation, are discussed. Computational tests on pathological test cases from adaptive finite element methods show the performance of the technique. C1 [Brune, Peter R.] Argonne Natl Lab, Div Math & Comp Sci, Argonne, IL 60439 USA. [Knepley, Matthew G.] Univ Chicago, Computat Inst, Chicago, IL 60637 USA. [Scott, L. Ridgway] Univ Chicago, Dept Comp Sci, Chicago, IL 60637 USA. RP Brune, PR (reprint author), Argonne Natl Lab, Div Math & Comp Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM brune@mcs.anl.gov; knepley@ci.uchicago.edu; ridg@uchicago.edu RI Knepley, Matthew/C-1094-2015 OI Knepley, Matthew/0000-0002-2292-0735 FU NSF [DMS-0920960]; Office of Advanced Scientific Computing Research, Office of Science, U.S. Department of Energy [DE-AC02-06CH11357] FX The work of the first two authors was partially supported by NSF grant DMS-0920960.; This author's work was supported by the Office of Advanced Scientific Computing Research, Office of Science, U.S. Department of Energy, under contract DE-AC02-06CH11357. NR 40 TC 4 Z9 4 U1 1 U2 7 PU SIAM PUBLICATIONS PI PHILADELPHIA PA 3600 UNIV CITY SCIENCE CENTER, PHILADELPHIA, PA 19104-2688 USA SN 1064-8275 EI 1095-7197 J9 SIAM J SCI COMPUT JI SIAM J. Sci. Comput. PY 2013 VL 35 IS 1 BP A173 EP A191 DI 10.1137/110827077 PG 19 WC Mathematics, Applied SC Mathematics GA 098UQ UT WOS:000315575000008 ER PT J AU Almgren, AS Aspden, AJ Bell, JB Minion, ML AF Almgren, A. S. Aspden, A. J. Bell, J. B. Minion, M. L. TI ON THE USE OF HIGHER-ORDER PROJECTION METHODS FOR INCOMPRESSIBLE TURBULENT FLOW SO SIAM JOURNAL ON SCIENTIFIC COMPUTING LA English DT Article DE higher-order projection; auxiliary formulation; spectral deferred correction ID NAVIER-STOKES EQUATIONS; BOUNDARY-VALUE-PROBLEMS; RUNGE-KUTTA METHODS; SEMIIMPLICIT NUMERICAL SCHEME; MACH NUMBER COMBUSTION; DIFFERENTIAL-EQUATIONS; DEFERRED CORRECTIONS; REACTING FLOW; GAS-DYNAMICS; SIMULATIONS AB An important issue in the development of higher-order methods for incompressible flow is how they perform when the flow is turbulent. A useful diagnostic of a method for turbulent flow is the minimum resolution that is required to adequately resolve the turbulent energy cascade at a given Reynolds number. In this paper, we present careful numerical experiments to assess the utility of higher-order numerical methods based on this metric. We first introduce a numerical method for the incompressible Navier-Stokes equations based on fourth-order discretizations in both space and time. The method is based on an auxiliary variable formulation and combines fourth-order finite volume differencing with a semi-implicit spectral deferred correction temporal integration scheme. We also introduce, for comparison purposes, versions based on second-order spatial and/or temporal discretizations. We demonstrate that for smooth problems, each of the methods exhibits the expected order of convergence in time and space. We next examine the behavior of these schemes on prototypical turbulent flows; in particular, we consider homogeneous isotropic turbulence in which long wavelength forcing is used to maintain the overall level of turbulent intensity. We provide comparisons of the fourth-order method with the comparable second-order method as well as with a second-order semi-implicit projection method based on a shock-capturing discretization. The results demonstrate that, for a given Reynolds number, the fourth-order scheme leads to dramatic reduction in the required resolution relative to either of the second-order schemes. In addition, the resolution requirements appear to be reasonably well predicted by scaling relationships based on dimensional analysis, providing a characterization of resolution requirements as a function of Reynolds number. C1 [Almgren, A. S.; Aspden, A. J.; Bell, J. B.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Ctr Computat Sci & Engn, Berkeley, CA 94720 USA. [Aspden, A. J.] Univ Portsmouth, Sch Engn, Portsmouth PO1 3DJ, Hants, England. [Minion, M. L.] Univ N Carolina, Dept Math, Chapel Hill, NC 27599 USA. RP Almgren, AS (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Ctr Computat Sci & Engn, Berkeley, CA 94720 USA. EM asalmgren@lbl.gov; andrew.aspden@port.ac.uk; jbbell@lbl.gov; min-ion@email.unc.edu RI Aspden, Andy/A-7391-2017 OI Aspden, Andy/0000-0002-2970-4824 FU Applied Mathematics Program of the DOE Office of Advanced Scientific Computing Research under the U.S. Department of Energy [DE-AC02-05CH11231]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; Alexander von Humboldt Foundation; DOE Office of Science, Office of Advanced Scientific Computing Research, Office of Mathematics, Information, and Computational Sciences, Applied Mathematical Sciences Program [DE-SC0004011]; National Science Foundation [DMS-0854961] FX This work was supported by the Applied Mathematics Program of the DOE Office of Advanced Scientific Computing Research under the U.S. Department of Energy under contract DE-AC02-05CH11231. Simulations used resources at National Energy Research Scientific Computing Center (NERSC), which is supported by the Office of Science of the U.S. Department of Energy under contract DE-AC02-05CH11231. The U.S. Government retains a nonexclusive, royalty-free license to publish or reproduce the published form of this contribution, or allow others to do so, for U.S. Government purposes. Copyright is owned by SIAM to the extent not limited by these rights.; This author's work was supported by the Alexander von Humboldt Foundation, and the Director, DOE Office of Science, Office of Advanced Scientific Computing Research, Office of Mathematics, Information, and Computational Sciences, Applied Mathematical Sciences Program, under contract DE-SC0004011, and the National Science Foundation under contract DMS-0854961. NR 39 TC 4 Z9 4 U1 0 U2 9 PU SIAM PUBLICATIONS PI PHILADELPHIA PA 3600 UNIV CITY SCIENCE CENTER, PHILADELPHIA, PA 19104-2688 USA SN 1064-8275 J9 SIAM J SCI COMPUT JI SIAM J. Sci. Comput. PY 2013 VL 35 IS 1 BP B25 EP B42 DI 10.1137/110829386 PG 18 WC Mathematics, Applied SC Mathematics GA 098UQ UT WOS:000315575000025 ER PT J AU Bock, N Challacombe, M AF Bock, Nicolas Challacombe, Matt TI AN OPTIMIZED SPARSE APPROXIMATE MATRIX MULTIPLY FOR MATRICES WITH DECAY SO SIAM JOURNAL ON SCIENTIFIC COMPUTING LA English DT Article DE sparse approximate matrix multiply; sparse linear algebra; SpAMM; reduced complexity algorithm; quantum chemistry; N-body; matrices with decay ID LINEAR SCALING COMPUTATION; FAST GAUSS TRANSFORM; ELECTRONIC-STRUCTURE CALCULATIONS; ADAPTIVE MESH REFINEMENT; CONSISTENT-FIELD THEORY; HIERARCHICALLY SEMISEPARABLE REPRESENTATIONS; EXCHANGE-CORRELATION MATRIX; DENSITY-FUNCTIONAL THEORY; FOCK MATRIX; CONQUER APPROACH AB We present an optimized single-precision implementation of the sparse approximate matrix multiply (SpAMM) [M. Challacombe and N. Bock, arXiv 1011.3534, 2010], a fast algorithm for matrix-matrix multiplication for matrices with decay that achieves an O(n log n) computational complexity with respect to matrix dimension n. We find that the max norm of the error achieved with a SpAMM tolerance below 2 x 10(-8) is lower than that of the single-precision general matrix-matrix multiply (SGEMM) for dense quantum chemical matrices, while outperforming SGEMM with a crossover already for small matrices (n similar to 1000). Relative to naive implementations of SpAMM using Intel's Math Kernel Library or AMD's Core Math Library, our optimized version is found to be significantly faster. Detailed performance comparisons are made for quantum chemical matrices with differently structured sub-blocks. Finally, we discuss the potential of improved hardware prefetch to yield 2x to 3x speedups. C1 [Bock, Nicolas; Challacombe, Matt] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87544 USA. RP Bock, N (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87544 USA. EM nbock@lanl.gov; mchalla@lanl.gov FU U.S. Department of Energy [DE-AC52-06NA25396]; LDRD-ER [20110230ER] FX Submitted to the journal's High-Performance Computing section March 21, 2012; accepted for publication (in revised form) November 30, 2012; published electronically January 29, 2013. This work was supported by the U.S. Department of Energy under contract DE-AC52-06NA25396 and LDRD-ER grant 20110230ER. This paper was released under LA-UR 11-06091. NR 145 TC 8 Z9 8 U1 3 U2 10 PU SIAM PUBLICATIONS PI PHILADELPHIA PA 3600 UNIV CITY SCIENCE CENTER, PHILADELPHIA, PA 19104-2688 USA SN 1064-8275 EI 1095-7197 J9 SIAM J SCI COMPUT JI SIAM J. Sci. Comput. PY 2013 VL 35 IS 1 BP C72 EP C98 DI 10.1137/120870761 PG 27 WC Mathematics, Applied SC Mathematics GA 098UQ UT WOS:000315575000041 ER PT S AU Tylutki, M Dziarmaga, J Zurek, WH AF Tylutki, Marek Dziarmaga, Jacek Zurek, Wojciech H. GP IOP TI Dynamics of the Mott Insulator to Superfluid quantum phase transition in the truncated Wigner approximation SO 21ST INTERNATIONAL LASER PHYSICS WORKSHOP SE Journal of Physics Conference Series LA English DT Proceedings Paper CT 21st International Laser Physics Workshop CY JUL 23-27, 2012 CL Calgary, CANADA ID BOSE-EINSTEIN CONDENSATE; COSMOLOGICAL EXPERIMENTS; FIELD; RELAXATION; STRINGS; GASES AB The quantum phase transition from the Mott insulator state to the superfluid in the Bose-Hubbard model is investigated. We research one, two and three dimensional lattices in the truncated Wigner approximation. We compute both kinetic and potential energy and they turn out to have a power law behaviour as a function of the transition rate, with the power equal to 1/3. The same applies to the total energy in a system with a harmonic trap, which is usually present in the experimental set-up. These observations are in agreement with the experiment of [8], where such scalings were also observed and the power of the decay was numerically close to 1/3. The results confirm the Kibble-Zurek (adiabatic-impulse-adiabatic approximation) scenario for this transition. C1 [Tylutki, Marek; Dziarmaga, Jacek] Jagiellonian Univ, Inst Phys, Reymonta 4, PL-30059 Krakow, Poland. [Zurek, Wojciech H.] Los Alamos Natl Lab, Div Theor, Los Alamos, NM 87545 USA. RP Tylutki, M (reprint author), Jagiellonian Univ, Inst Phys, Reymonta 4, PL-30059 Krakow, Poland. EM marek.tylutki@uj.edu.pl FU NCN [2011/01/B/ST3/00512]; PL-Grid Infrastructure FX This work was supported in part by the NCN grant 2011/01/B/ST3/00512 (JD and MT) and the PL-Grid Infrastructure (MT). NR 60 TC 2 Z9 2 U1 0 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA DIRAC HOUSE, TEMPLE BACK, BRISTOL BS1 6BE, ENGLAND SN 1742-6588 J9 J PHYS CONF SER PY 2013 VL 414 AR 012029 DI 10.1088/1742-6596/414/1/012029 PG 14 WC Optics; Physics, Applied SC Optics; Physics GA BDW69 UT WOS:000315404300029 ER PT S AU Sarret, G Smits, EAHP Michel, HC Isaure, MP Zhao, FJ Tappero, R AF Sarret, G. Smits, E. A. H. Pilon Michel, H. Castillo Isaure, M. P. Zhao, F. J. Tappero, R. BE Sparks, DL TI Use of Synchrotron-Based Techniques to Elucidate Metal Uptake and Metabolism in Plants SO ADVANCES IN AGRONOMY, VOL 119 SE Advances in Agronomy LA English DT Review; Book Chapter ID RAY-ABSORPTION SPECTROSCOPY; PLASMA-MASS-SPECTROMETRY; HYPERACCUMULATOR PTERIS-VITTATA; LA-ICP-MS; SCANNING-ELECTRON-MICROSCOPY; EDGE COMPUTED MICROTOMOGRAPHY; PRINCIPAL COMPONENT ANALYSIS; CAERULESCENS GANGES ECOTYPE; CUCUMBER CUCUMIS-SATIVUS; MESQUITE PROSOPIS SPP. AB Synchrotron techniques have become key components of the toolbox for studying the mechanisms involved in metal(loid) uptake and metabolism in plants. Most widely used techniques in this field include micro-X-ray fluorescence (mu XRF) for imaging the distribution of elements in plant tissues and cells and quantifying them, and X-ray absorption spectroscopy (XAS) for determining their chemical forms. Recent advances in terms of spatial resolution, sensitivity and versatility of the sample environment have opened new perspectives for the study of trace elements at the micro- and nanoscale with a minimal perturbation of the sample. Sample conditioning remains a key issue for the study of metals in plants. Cryogenic sample environments allow work on hydrated systems, with a limited risk of metal remobilization and changes in speciation. Still, radiation damage should be monitored carefully, especially for high-flux spectrometers. In addition, progress in software for data analysis has facilitated data mining and integration of results from various techniques. This chapter presents the principle and the basics of data analysis for mu XRF imaging and tomography, XAS and micro-Fourier transform infrared spectromicroscopy (mu FTIR). Major results obtained on Ni, Cd, Zn, Se, As, Cu, Mn and nanoparticles in hyperaccumulating and nonaccumulating plants are presented. Complementary approaches including histochemical techniques, micro and nanoscopic techniques using electron- or ion beams, and laser ablation coupled with inductively coupled plasma mass spectrometry (ICP-MS) are also presented, and key results reviewed. Finally, there is also great interest in coupling synchrotron techniques, which is possible on more and more beamlines, and also in coupling synchrotron techniques with other approaches such as the ones mentioned above; perspectives in this area are discussed. C1 [Sarret, G.] Univ Grenoble 1, CNRS, ISTerre, Inst Sci Terre, Grenoble, France. [Smits, E. A. H. Pilon] Colorado State Univ, Dept Biol, Ft Collins, CO 80523 USA. [Michel, H. Castillo] European Synchrotron Radiat Facil, F-38043 Grenoble, France. [Isaure, M. P.] Univ Pau & Pays Adour, CNRS, LCABIE, Inst Sci Analyt & Physicochim Environm & Mat, Pau 09, France. [Zhao, F. J.] Nanjing Agr Univ, Coll Resources & Environm Sci, Nanjing, Peoples R China. [Zhao, F. J.] Rothamsted Res, Harpenden, Herts, England. [Tappero, R.] Brookhaven Natl Lab, Photon Sci Dept, NSLS, Upton, NY 11973 USA. RP Sarret, G (reprint author), Univ Grenoble 1, CNRS, ISTerre, Inst Sci Terre, Grenoble, France. EM geraldine.sarret@ujf-grenoble.fr RI Beamline, FAME/G-9313-2012; Zhao, Fang-Jie/A-8339-2008; Sarret, Geraldine/I-2797-2016 OI Zhao, Fang-Jie/0000-0002-0164-169X; NR 307 TC 31 Z9 32 U1 11 U2 192 PU ELSEVIER ACADEMIC PRESS INC PI SAN DIEGO PA 525 B STREET, SUITE 1900, SAN DIEGO, CA 92101-4495 USA SN 0065-2113 BN 978-0-12-407247-3 J9 ADV AGRON JI Adv. Agron. PY 2013 VL 119 BP 1 EP + DI 10.1016/B978-0-12-407247-3.00001-9 PG 20 WC Agronomy SC Agriculture GA BDW92 UT WOS:000315471300001 ER PT J AU Diwan, M Edgecock, R Hasegawa, T Patzak, T Shiozawa, M Strait, J AF Diwan, Milind Edgecock, Rob Hasegawa, Takuya Patzak, Thomas Shiozawa, Masato Strait, Jim TI Future Long-Baseline Neutrino Facilities and Detectors SO ADVANCES IN HIGH ENERGY PHYSICS LA English DT Review ID LIQUID SCINTILLATOR DETECTOR; BEAM AB We review the ongoing effort in the US, Japan, and Europe of the scientific community to study the location and the detector performance of the next-generation long-baseline neutrino facility. For many decades, research on the properties of neutrinos and the use of neutrinos to study the fundamental building blocks of matter has unveiled new, unexpected laws of nature. Results of neutrino experiments have triggered a tremendous amount of development in theory: theories beyond the standard model or at least extensions of it and development of the standard solar model and modeling of supernova explosions as well as the development of theories to explain the matter-antimatter asymmetry in the universe. Neutrino physics is one of the most dynamic and exciting fields of research in fundamental particle physics and astrophysics. The next-generation neutrino detector will address two aspects: fundamental properties of the neutrino like mass hierarchy, mixing angles, and the CP phase, and low-energy neutrino astronomy with solar, atmospheric, and supernova neutrinos. Such a new detector naturally allows for major improvements in the search for nucleon decay. A next-generation neutrino observatory needs a huge, megaton scale detector which in turn has to be installed in a new, international underground laboratory, capable of hosting such a huge detector. C1 [Diwan, Milind] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Edgecock, Rob] Univ Huddersfield, Didcot OX11 0QX, Oxon, England. [Edgecock, Rob] STFC Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Hasegawa, Takuya] High Energy Accelerator Res Org KEK, Tsukuba, Ibaraki 3050801, Japan. [Patzak, Thomas] Univ Paris Diderot, Observ Paris, CNRS IN2P3, CEA Irfu, F-75205 Paris 13, France. [Shiozawa, Masato] Univ Tokyo, Inst Cosm Ray Res, Kamioka Observ, Gifu 5061205, Japan. [Strait, Jim] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. RP Patzak, T (reprint author), Univ Paris Diderot, Observ Paris, CNRS IN2P3, CEA Irfu, 10 Rue Alice Domon & Leonie Duquet, F-75205 Paris 13, France. EM patzak@apc.univ-paris7.fr FU European Commission [212343]; LAGUNA-LBNO [284518]; EUROnu [212372]; Japan Society for the Promotion of Science [23244058]; US Department of Energy FX The authors are grateful to the European Commission for the financial support of the project through the FP7 Design Studies LAGUNA (Project no. 212343), LAGUNA-LBNO (Project no. 284518), and EUROnu (Project no. 212372). The EC is not liable for any use that may be made of the information herein. They thank the French Centre National de Recherche Scientifique for the support of the project in form of the PICS. They are also grateful to the Japan Society for the Promotion of Science Grants-in-Aid for Scientific Research (Grant no. 23244058). This work was partially supported by the US Department of Energy. NR 74 TC 4 Z9 4 U1 0 U2 4 PU HINDAWI PUBLISHING CORPORATION PI NEW YORK PA 410 PARK AVENUE, 15TH FLOOR, #287 PMB, NEW YORK, NY 10022 USA SN 1687-7357 J9 ADV HIGH ENERGY PHYS JI Adv. High. Energy Phys. PY 2013 AR 460123 DI 10.1155/2013/460123 PG 35 WC Physics, Particles & Fields SC Physics GA 102VN UT WOS:000315872600001 ER PT J AU Howcroft, TK Campisi, J Louis, GB Smith, MT Wise, B Wyss-Coray, T Augustine, AD McElhaney, JE Kohanski, R Sierra, F AF Howcroft, T. Kevin Campisi, Judith Louis, Germaine Buck Smith, Martyn T. Wise, Bradley Wyss-Coray, Tony Augustine, Alison Deckhut McElhaney, Janet E. Kohanski, Ron Sierra, Felipe TI The role of inflammation in age-related disease SO AGING-US LA English DT Article AB The National Institutes of Health (NIH) Geroscience Interest Group (GSIG) sponsored workshop, The Role of Inflammation in Age-Related Disease, was held September 6th-7th, 2012 in Bethesda, MD. It is now recognized that a mild pro-inflammatory state is correlated with the major degenerative diseases of the elderly. The focus of the workshop was to better understand the origins and consequences of this low level chronic inflammation in order to design appropriate interventional studies aimed at improving healthspan. Four sessions explored the intrinsic, environmental exposures and immune pathways by which chronic inflammation are generated, sustained, and lead to age-associated diseases. At the conclusion of the workshop recommendations to accelerate progress toward understanding the mechanistic bases of chronic disease were identified. C1 [Howcroft, T. Kevin] NCI, Div Canc Biol, NIH, Bethesda, MD 20892 USA. [Campisi, Judith] Buck Inst Res Aging, Novato, CA 94945 USA. [Campisi, Judith] Lawrence Berkeley Natl Lab, Berkeley, CA 94702 USA. [Louis, Germaine Buck] NICHD, Off Director, NIH, Bethesda, MD 20892 USA. [Smith, Martyn T.] Univ Calif Berkeley, Div Environm Hlth Sci, Berkeley, CA 94720 USA. [Wise, Bradley] NIA, Div Neurosci, NIH, Bethesda, MD 20892 USA. [Wyss-Coray, Tony] Stanford Univ, Dept Neurol & Neurol Sci, Sch Med, Stanford, CA 94305 USA. [Augustine, Alison Deckhut] NIAID, Div Allergy Immunol & Transplantat, NIH, Bethesda, MD 20892 USA. [McElhaney, Janet E.] Adv Med Res Inst Canada, Sudbury, ON P3E 5J1, Canada. [Kohanski, Ron; Sierra, Felipe] NIA, Div Aging Biol, NIH, Bethesda, MD 20892 USA. RP Howcroft, TK (reprint author), NCI, Div Canc Biol, NIH, Bethesda, MD 20892 USA. EM Howcrofk@mail.nih.gov; Kohanskir@mail.nih.gov; sierraf@mail.nih.gov OI Buck Louis, Germaine/0000-0002-1774-4490 FU NIEHS NIH HHS [P42 ES004705] NR 0 TC 50 Z9 53 U1 1 U2 5 PU IMPACT JOURNALS LLC PI ALBANY PA 6211 TIPTON HOUSE, STE 6, ALBANY, NY 12203 USA SN 1945-4589 J9 AGING-US JI Aging-US PD JAN PY 2013 VL 5 IS 1 BP 84 EP 93 PG 10 WC Cell Biology SC Cell Biology GA 104HH UT WOS:000315982300007 PM 23474627 ER PT J AU Lanekoff, I Geydebrekht, O Pinchuk, GE Konopka, AE Laskin, J AF Lanekoff, Ingela Geydebrekht, Oleg Pinchuk, Grigoriy E. Konopka, Allan E. Laskin, Julia TI Spatially resolved analysis of glycolipids and metabolites in living Synechococcus sp PCC 7002 using nanospray desorption electrospray ionization SO ANALYST LA English DT Article ID IMAGING MASS-SPECTROMETRY; SURFACE SAMPLING PROBE; BLUE-GREEN-ALGAE; BACILLUS-SUBTILIS; PHOSPHATE SYNTHASE; MICROBIAL ECOLOGY; FATTY-ACIDS; IDENTIFICATION; TEMPERATURE; EXPRESSION AB Microorganisms release a diversity of organic compounds that couple interspecies metabolism, enable communication, or provide benefits to other microbes. Increased knowledge of microbial metabolite production will contribute to understanding of the dynamic microbial world and can potentially lead to new developments in drug discovery, biofuel production, and clinical research. Nanospray desorption electrospray ionization (nano-DESI) is an ambient ionization technique that enables detailed chemical characterization of molecules from a specific location on a surface without special sample pretreatment. Due to its ambient nature, living bacterial colonies growing on agar plates can be rapidly analyzed without affecting the viability of the colony. In this study we demonstrate for the first time the utility of nano-DESI for spatial profiling of chemical gradients generated by microbial communities on agar plates. We found that despite the high salt content of the agar used in this study (similar to 350 mM), nano-DESI analysis enables detailed characterization of metabolites produced by the Synechococcus sp. PCC 7002 colonies. High resolution mass spectrometry and MS/MS analysis of the living Synechococcus sp. PCC 7002 colonies allowed us to detect metabolites and lipids on the colony and on the surrounding agar, and confirm their identities. High sensitivity of nano-DESI enabled identification of several glycolipids that have not been previously reported by extracting the cells using conventional methods. Spatial profiling demonstrated that a majority of lipids and metabolites were localized on the colony while sucrose and glucosylglycerol, an osmoprotective compound produced by cyanobacteria, were secreted onto agar. Furthermore, we demonstrated that the chemical gradients of sucrose and glucosylglycerol on agar depend on the age of the colony. The methodology presented in this study will facilitate future studies focused on molecular-level characterization of interactions between bacterial colonies. C1 [Lanekoff, Ingela; Laskin, Julia] Pacific NW Natl Lab, Div Chem & Mat Sci, Richland, WA 99352 USA. [Geydebrekht, Oleg; Pinchuk, Grigoriy E.; Konopka, Allan E.] Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99352 USA. RP Lanekoff, I (reprint author), Pacific NW Natl Lab, Div Chem & Mat Sci, POB 999,K8-88, Richland, WA 99352 USA. EM Ingela.Lanekoff@pnnl.gov; Julia.Laskin@pnnl.gov RI Laskin, Julia/H-9974-2012 OI Laskin, Julia/0000-0002-4533-9644 FU DOE's Office of Biological and Environmental Research FX The research described in this paper is part of the Chemical Imaging Initiative at Pacific Northwest National Laboratory (PNNL). It was conducted under the Laboratory Directed Research and Development Program at PNNL, a multiprogram national laboratory operated by Battelle for the U.S. Department of Energy (DOE). The work was performed using EMSL, a national scientific user facility sponsored by the DOE's Office of Biological and Environmental Research and located at PNNL. NR 74 TC 27 Z9 27 U1 6 U2 100 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 0003-2654 J9 ANALYST JI Analyst PY 2013 VL 138 IS 7 BP 1971 EP 1978 DI 10.1039/c3an36716a PG 8 WC Chemistry, Analytical SC Chemistry GA 099DA UT WOS:000315598500008 PM 23392077 ER PT J AU Belikov, DA Maksyutov, S Krol, M Fraser, A Rigby, M Bian, H Agusti-Panareda, A Bergmann, D Bousquet, P Cameron-Smith, P Chipperfield, MP Fortems-Cheiney, A Gloor, E Haynes, K Hess, P Houweling, S Kawa, SR Law, RM Loh, Z Meng, L Palmer, PI Patra, PK Prinn, RG Saito, R Wilson, C AF Belikov, D. A. Maksyutov, S. Krol, M. Fraser, A. Rigby, M. Bian, H. Agusti-Panareda, A. Bergmann, D. Bousquet, P. Cameron-Smith, P. Chipperfield, M. P. Fortems-Cheiney, A. Gloor, E. Haynes, K. Hess, P. Houweling, S. Kawa, S. R. Law, R. M. Loh, Z. Meng, L. Palmer, P. I. Patra, P. K. Prinn, R. G. Saito, R. Wilson, C. TI Off-line algorithm for calculation of vertical tracer transport in the troposphere due to deep convection SO ATMOSPHERIC CHEMISTRY AND PHYSICS LA English DT Article ID GENERAL-CIRCULATION MODEL; OBSERVED RADON PROFILES; CUMULUS CONVECTION; ATMOSPHERIC TRANSPORT; CLIMATE SIMULATIONS; METEOROLOGICAL DATA; CLOUD ENSEMBLE; PRECIPITATION; RN-222; PARAMETERIZATION AB A modified cumulus convection parametrisation scheme is presented. This scheme computes the mass of air transported upward in a cumulus cell using conservation of moisture and a detailed distribution of convective precipitation provided by a reanalysis dataset. The representation of vertical transport within the scheme includes entrainment and detrainment processes in convective updrafts and downdrafts. Output from the proposed parametrisation scheme is employed in the National Institute for Environmental Studies (NIES) global chemical transport model driven by JRA-25/JCDAS reanalysis. The simulated convective precipitation rate and mass fluxes are compared with observations and reanalysis data. A simulation of the short-lived tracer Rn-222 is used to further evaluate the performance of the cumulus convection scheme. Simulated distributions of Rn-222 are evaluated against observations at the surface and in the free troposphere, and compared with output from models that participated in the TransCom-CH4 Transport Model Intercomparison. From this comparison, we demonstrate that the proposed convective scheme in general is consistent with observed and modeled results. C1 [Belikov, D. A.; Maksyutov, S.] Natl Inst Environm Studies, Ctr Global Environm Res, Tsukuba, Ibaraki 3058506, Japan. [Belikov, D. A.] Natl Inst Polar Res, Div Polar Res, Tachikawa, Tokyo 1908518, Japan. [Krol, M.; Houweling, S.] SRON Netherlands Inst Space Res, NL-3584 CA Utrecht, Netherlands. [Krol, M.; Houweling, S.] Inst Marine & Atmospher Res Utrecht IMAU, NL-3584 CC Utrecht, Netherlands. [Krol, M.] Univ Wageningen & Res Ctr, NL-6708 PB Wageningen, Netherlands. [Fraser, A.; Palmer, P. I.] Univ Edinburgh, Sch Geosci, Edinburgh EH9 3JN, Midlothian, Scotland. [Rigby, M.] Univ Bristol, Bristol, Avon, England. [Bian, H.; Kawa, S. R.] NASA, Goddard Space Flight Ctr, Goddard Earth Sci & Technol Ctr, Greenbelt, MD 20771 USA. [Agusti-Panareda, A.] ECMWF, Reading RG2 9AX, Berks, England. [Bergmann, D.; Cameron-Smith, P.] Lawrence Livermore Natl Lab, Atmospher Earth & Energy Div, Livermore, CA 94550 USA. [Bousquet, P.; Fortems-Cheiney, A.] Univ Versailles St Quentin Yvelines UVSQ, GIF YVETTE, Gif Sur Yvette, France. [Chipperfield, M. P.; Gloor, E.; Wilson, C.] Univ Leeds, Sch Earth & Environm, Inst Climate & Atmospher Sci, Leeds LS2 9JT, W Yorkshire, England. [Haynes, K.] Colorado State Univ, Dept Atmospher Sci, Ft Collins, CO 80523 USA. [Haynes, K.; Law, R. M.; Loh, Z.] CSIRO Marine & Atmospher Res, Ctr Australian Weather & Climate Res, Aspendale, Vic 3195, Australia. [Hess, P.] Cornell Univ, Ithaca, NY 14850 USA. [Meng, L.] Western Michigan Univ, Dept Geog, Kalamazoo, MI 49008 USA. [Meng, L.] Western Michigan Univ, Environm Studies Program, Kalamazoo, MI 49008 USA. [Patra, P. K.; Saito, R.] Res Inst Global Change JAMSTEC, Yokohama, Kanagawa 2360001, Japan. [Prinn, R. G.] MIT, Ctr Global Change Sci, Cambridge, MA 02139 USA. RP Belikov, DA (reprint author), Natl Inst Environm Studies, Ctr Global Environm Res, 16-2 Onogawa, Tsukuba, Ibaraki 3058506, Japan. EM dmitry.belikov@nies.go.jp RI Cameron-Smith, Philip/E-2468-2011; Fraser, Annemarie/D-3874-2012; Belikov, Dmitry/I-9877-2016; Rigby, Matthew/A-5555-2012; Bergmann, Daniel/F-9801-2011; Law, Rachel/A-1969-2012; Meng, Lei/H-5253-2013; Chipperfield, Martyn/H-6359-2013; Kawa, Stephan/E-9040-2012; Krol, Maarten/E-3414-2013; Palmer, Paul/F-7008-2010; Maksyutov, Shamil/G-6494-2011; Hess, Peter/M-3145-2015 OI Wilson, Chris/0000-0001-8494-0697; Cameron-Smith, Philip/0000-0002-8802-8627; Rigby, Matthew/0000-0002-2020-9253; Bergmann, Daniel/0000-0003-4357-6301; Law, Rachel/0000-0002-7346-0927; Chipperfield, Martyn/0000-0002-6803-4149; Maksyutov, Shamil/0000-0002-1200-9577; Hess, Peter/0000-0003-2439-3796 NR 72 TC 7 Z9 7 U1 0 U2 18 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1680-7316 EI 1680-7324 J9 ATMOS CHEM PHYS JI Atmos. Chem. Phys. PY 2013 VL 13 IS 3 BP 1093 EP 1114 DI 10.5194/acp-13-1093-2013 PG 22 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 096LR UT WOS:000315406100001 ER PT J AU Akagi, SK Yokelson, RJ Burling, IR Meinardi, S Simpson, I Blake, DR McMeeking, GR Sullivan, A Lee, T Kreidenweis, S Urbanski, S Reardon, J Griffith, DWT Johnson, TJ Weise, DR AF Akagi, S. K. Yokelson, R. J. Burling, I. R. Meinardi, S. Simpson, I. Blake, D. R. McMeeking, G. R. Sullivan, A. Lee, T. Kreidenweis, S. Urbanski, S. Reardon, J. Griffith, D. W. T. Johnson, T. J. Weise, D. R. TI Measurements of reactive trace gases and variable O-3 formation rates in some South Carolina biomass burning plumes SO ATMOSPHERIC CHEMISTRY AND PHYSICS LA English DT Article ID TRANSFORM INFRARED-SPECTROSCOPY; SECONDARY ORGANIC AEROSOL; FIRE EMISSIONS EXPERIMENT; UNITED-STATES; LABORATORY MEASUREMENTS; PARTICLE EMISSIONS; TROPICAL FOREST; ATMOSPHERIC CHEMISTRY; CARBONYL SULFIDE; PRESCRIBED FIRES AB In October-November 2011 we measured trace gas emission factors from seven prescribed fires in South Carolina (SC), US, using two Fourier transform infrared spectrometer (FTIR) systems and whole air sampling (WAS) into canisters followed by gas-chromatographic analysis. A total of 97 trace gas species were quantified from both airborne and ground-based sampling platforms, making this one of the most detailed field studies of fire emissions to date. The measurements include the first emission factors for a suite of monoterpenes produced by heating vegetative fuels during field fires. The first quantitative FTIR observations of limonene in smoke are reported along with an expanded suite of monoterpenes measured by WAS including alpha-pinene, beta-pinene, limonene, camphene, 4-carene, and myrcene. The known chemistry of the monoterpenes and their measured abundance of 0.4-27.9% of non-methane organic compounds (NMOCs) and similar to 21% of organic aerosol (mass basis) suggests that they impacted secondary formation of ozone (O-3), aerosols, and small organic trace gases such as methanol and formaldehyde in the sampled plumes in the first few hours after emission. The variability in the initial terpene emissions in the SC fire plumes was high and, in general, the speciation of the initially emitted gas-phase NMOCs was 13-195% different from that observed in a similar study in nominally similar pine forests in North Carolina similar to 20 months earlier. It is likely that differences in stand structure and environmental conditions contributed to the high variability observed within and between these studies. Similar factors may explain much of the variability in initial emissions in the literature. The Delta HCN/Delta CO emission ratio, however, was found to be fairly consistent with previous airborne fire measurements in other coniferous-dominated ecosystems, with the mean for these studies being 0.90+/-0.06 %, further confirming the value of HCN as a biomass burning tracer. The SC results also support an earlier finding that C3C4 alkynes may be of use as biomass burning indicators on the time-scale of hours to a day. It was possible to measure the downwind chemical evolution of the plume on four of the fires and significant O-3 formation (Delta O-3/Delta CO from 1090 %) occurred in all of these plumes within two hours. The slowest O-3 production was observed on a cloudy day with low co-emission of NOx. The fastest O-3 production was observed on a sunny day when the downwind plume almost certainly incorporated significant additional NOx by passing over the Columbia, SC metropolitan area. Due to rapid plume dilution, it was only possible to acquire high-quality downwind data for two other trace gas species (formaldehyde and methanol) during two of the fires. In all four of these cases, significant increases in formaldehyde and methanol were observed in < 2 h. This is likely the first direct observation of post-emission methanol production in biomass burning plumes. Post-emission production of methanol does not always happen in young biomass burning plumes, and its occurrence in this study could have involved terpene precursors to a significant extent. C1 [Akagi, S. K.; Yokelson, R. J.; Burling, I. R.] Univ Montana, Dept Chem, Missoula, MT 59812 USA. [Meinardi, S.; Simpson, I.; Blake, D. R.] Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA. [McMeeking, G. R.; Sullivan, A.; Lee, T.; Kreidenweis, S.] Colorado State Univ, Dept Atmospher Sci, Ft Collins, CO 80523 USA. [Urbanski, S.; Reardon, J.] US Forest Serv, USDA, Rocky Mt Res Stn, Fire Sci Lab, Missoula, MT 59808 USA. [Griffith, D. W. T.] Univ Wollongong, Dept Chem, Wollongong, NSW 2500, Australia. [Johnson, T. J.] Pacific NW Natl Lab, Richland, WA 99354 USA. [Weise, D. R.] US Forest Serv, USDA, Pacific Southwest Res Stn, Forest Fire Lab, Riverside, CA 92507 USA. RP Yokelson, RJ (reprint author), Univ Montana, Dept Chem, Missoula, MT 59812 USA. EM bob.yokelson@umontana.edu RI Yokelson, Robert/C-9971-2011; Kreidenweis, Sonia/E-5993-2011 OI Yokelson, Robert/0000-0002-8415-6808; Kreidenweis, Sonia/0000-0002-2561-2914 FU Strategic Environmental Research and Development Program (SERDP) [RC-1649, 08JV11272166039]; Joint Fire Science Program [11-1-5-12, 08-1-6-09]; NSF [ATM 0513055] FX This work was supported by the Strategic Environmental Research and Development Program (SERDP) project RC-1649 and administered partly through Forest Service Research Joint Venture Agreement 08JV11272166039, and we thank the sponsors for their support. CSU was supported by Joint Fire Science Program grant # 11-1-5-12. Shawn Urbanski and some of the Twin Otter flight hours were supported by Joint Fire Science Program grant # 08-1-6-09. We appreciate the efforts of Aaron Sparks and Signe Leirfallom to measure the consumption of wildland fuels for this study. Adaptation of the USFS Twin Otter for research flights was supported primarily by NSF grant ATM 0513055. Special thanks to our pilot Bill Mank and Twin Otter mechanic Steve Woods. We thank Holly Eissinger for constructing maps of Fort Jackson flight tracks, hot spots, and fire locations shown in Figs. 2, 3, 4. We greatly appreciate the collaboration and efforts of John Maitland and forestry staff at Fort Jackson and we thank the Columbia dispatch office of the South Carolina Forestry Commission for assistance in locating fires to sample. NR 104 TC 50 Z9 50 U1 2 U2 75 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1680-7316 EI 1680-7324 J9 ATMOS CHEM PHYS JI Atmos. Chem. Phys. PY 2013 VL 13 IS 3 BP 1141 EP 1165 DI 10.5194/acp-13-1141-2013 PG 25 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 096LR UT WOS:000315406100004 ER PT J AU Strack, G Luckarift, HR Sizemore, SR Nichols, RK Farrington, KE Wu, PK Atanassov, P Biffinger, JC Johnson, GR AF Strack, Guinevere Luckarift, Heather R. Sizemore, Susan R. Nichols, Robert K. Farrington, Karen E. Wu, Peter K. Atanassov, Plamen Biffinger, Justin C. Johnson, Glenn R. TI Power generation from a hybrid biological fuel cell in seawater SO BIORESOURCE TECHNOLOGY LA English DT Article DE Microbial fuel cell; Shewanella oneidensis; Enzymatic fuel cell; Bilirubin oxidase; Multicopper oxidase ID ELECTRON-TRANSFER REACTIONS; SHEWANELLA-ONEIDENSIS; WASTE-WATER; REDUCTION; STABILITY; LACCASES; BIOFILMS; OXIDASES; SYSTEM; ANODES AB A hybrid biological fuel cell (HBFC) comprised of a microbial anode for lactate oxidation and an enzymatic cathode for oxygen reduction was constructed and then tested in a marine environment. Shewanella oneidensis DSP-10 was cultivated in laboratory medium and then fixed on a carbon felt electrode via a silica sol-gel process in order to catalyze anodic fuel cell processes. The cathode electrocatalyst was composed of bilirubin oxidase, fixed to a carbon nanotube electrode using a heterobifunctional cross linker, and then stabilized with a silica sol-gel coating. The anode and cathode half-cells provided operating potentials of -0.44 and 0.48 V, respectively (vs. Ag/AgCl). The HBFC maintained a reproducible open circuit voltage >0.7 V for 9 d in laboratory settings and sustained electrocatalytic activity for >24 h in open environment tests. Published by Elsevier Ltd. C1 [Strack, Guinevere; Luckarift, Heather R.; Sizemore, Susan R.; Nichols, Robert K.; Farrington, Karen E.; Johnson, Glenn R.] USAF, Microbiol & Appl Biochem Lab, Airbase Technol Div, Res Lab, Tyndall AFB, FL 32403 USA. [Strack, Guinevere] Oak Ridge Inst Sci & Engn, Oak Ridge, TN 37831 USA. [Luckarift, Heather R.; Sizemore, Susan R.; Nichols, Robert K.; Farrington, Karen E.] Universal Technol Corp, Dayton, OH 45432 USA. [Atanassov, Plamen] Univ New Mexico, Ctr Emerging Energy Technol, Albuquerque, NM 87131 USA. [Wu, Peter K.] Southern Oregon Univ, Dept Phys & Engn, Ashland, OR 97520 USA. [Biffinger, Justin C.] USN, Res Lab, Washington, DC 20375 USA. RP Johnson, GR (reprint author), USAF, Microbiol & Appl Biochem Lab, Airbase Technol Div, Res Lab, Tyndall AFB, FL 32403 USA. EM glenn.johnson.8@us.af.mil RI Atanassov, Plamen/G-4616-2011 FU US AFRL; Air Force Office of Scientific Research FX G. Strack was supported by an appointment to the Postgraduate Research Participation Program at the US AFRL administered by the Oak Ridge Institute for Science and Education through an inter-agency agreement between the US Department of Energy and USAFRL. The AFRL in-house research was supported in part by the Air Force Office of Scientific Research (Walt Kozumbo, Program Manager). NRL thank NRL/ONR BLK 6.2 funding for supporting the autonomous floating demonstration. The authors thank Marie Stephens (Mexico Beach, FL) for providing underwater photography, Kevin Randall and Jamie Vathis for use of watercraft, and Christopher Graeber (Integration Innovation, Inc., Huntsville, AL) for logistical support and open water test operations. NR 31 TC 10 Z9 10 U1 3 U2 43 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0960-8524 J9 BIORESOURCE TECHNOL JI Bioresour. Technol. PD JAN PY 2013 VL 128 BP 222 EP 228 DI 10.1016/j.biortech.2012.10.104 PG 7 WC Agricultural Engineering; Biotechnology & Applied Microbiology; Energy & Fuels SC Agriculture; Biotechnology & Applied Microbiology; Energy & Fuels GA 098JO UT WOS:000315545800031 PM 23196242 ER PT J AU Takaishi, S DeMarco, EJ Pellin, MJ Farha, OK Hupp, JT AF Takaishi, Shinya DeMarco, Erica J. Pellin, Michael J. Farha, Omar K. Hupp, Joseph T. TI Solvent-assisted linker exchange (SALE) and post-assembly metallation in porphyrinic metal-organic framework materials SO CHEMICAL SCIENCE LA English DT Article ID CATALYSIS; SOLIDS; MOF AB Using recently reported robust porphyrinic metal-organic framework (RPM) materials, we have examined the systematic exchange of pillaring linkers/struts as a means of accessing new versions of these materials. Dipyridyl-porphyrin Zn(II) (Zn-dipy) struts were successfully replaced by M-2-dipy (M-2 = 2H(+), Al(III), Sn(IV)), forming crystalline solid solutions of Zn(Zn1-xMx)-RPM in variable ratios. In addition, post-synthetic metallation was demonstrated using Zn2H-RPM, again with retention of crystallinity. We examined catalytic activity for an epoxide ring-opening reaction with a series of ZnM2-RPMs. The catalytic activity depends strongly on the identity of the metal ion present in the dipyridyl-porphyrin unit. C1 [Takaishi, Shinya; DeMarco, Erica J.; Pellin, Michael J.; Farha, Omar K.; Hupp, Joseph T.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Takaishi, Shinya; DeMarco, Erica J.; Pellin, Michael J.; Farha, Omar K.; Hupp, Joseph T.] Northwestern Univ, Int Inst Nanotechnol, Evanston, IL 60208 USA. [Takaishi, Shinya] Tohoku Univ, Grad Sch Sci, Dept Chem, Aoba Ku, Sendai, Miyagi 9808578, Japan. [Pellin, Michael J.; Hupp, Joseph T.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Takaishi, S (reprint author), Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. EM takaishi@mail.tains.tohoku.ac.jp; o-farha@northwestern.edu; j-hupp@northwestern.edu RI Hupp, Joseph/K-8844-2012; Pellin, Michael/B-5897-2008; Farha, Omar/B-5512-2014; Takaishi, Shinya/J-9006-2016 OI Hupp, Joseph/0000-0003-3982-9812; Pellin, Michael/0000-0002-8149-9768; Farha, Omar/0000-0002-9904-9845; FU DTRA [HDTRA1-09-10007]; U.S. Department of Energy, Office of Science, Office of Basic Energy Science [DE-SC0001059]; Tohoku University FX We gratefully acknowledge DTRA (grant no. HDTRA1-09-10007) for financial support of this project. SEM and EDX measurements were performed by E.J.D. We gratefully acknowledge the ANSER Center, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number DE-SC0001059, for support of her contribution to the study. S.T. thanks Tohoku University for its support during his sabbatical stay at Northwestern University. NR 33 TC 68 Z9 68 U1 18 U2 166 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2041-6520 J9 CHEM SCI JI Chem. Sci. PY 2013 VL 4 IS 4 BP 1509 EP 1513 DI 10.1039/c2sc21516k PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA 099CV UT WOS:000315597900014 ER PT J AU Cai, JJ Hay, BP Young, NJ Yang, XP Sessler, JL AF Cai, Jiajia Hay, Benjamin P. Young, Neil J. Yang, Xiaoping Sessler, Jonathan L. TI A pyrrole-based triazolium-phane with NH and cationic CH donor groups as a receptor for tetrahedral oxyanions that functions in polar media SO CHEMICAL SCIENCE LA English DT Article ID ION-PAIR RECEPTOR; 6-AMINOPICOLINIC ACID SUBUNITS; AZIDE-ALKYNE CYCLOADDITION; CLICK-CHEMISTRY; ANION RECOGNITION; MACROCYCLIC RECEPTOR; OLEFIN METATHESIS; AQUEOUS-SOLUTION; HYDROGEN-BONDS; CHLORIDE AB The pyrrole-based triazolium-phane 1(4+)center dot 4BF(4)(-) has been prepared via the tetraalkylation of a macrocycle originally prepared via click chemistry. It displays a high selectivity for tetrahedral oxyanions relative to various test monoanions and trigonal planar anions in mixed polar organic-aqueous media. This selectivity is solvent dependent and is less pronounced in acetonitrile. Theoretical calculations were carried out in with the chloride anion in an effort to understand the influence of solvent on the intrinsic hydrogen bonding ability of the donor groups (pyrrole N-H, benzene C-H and triazolium C-H). The host-guest interactions between receptor 1(4+)center dot 4BF(4)(-) and representative tetrahedral oxyanions were further analysed by H-1 NMR spectroscopy, and the findings proved consistent with the differences in the intrinsic strength of the various H-bond donor groups inferred from the electronic structure calculations carried out in methanol, namely that (CH)(+)-anion interactions are less important in an energetic sense than neutral CH-anion interactions in polar media. Single crystal X-ray diffraction analyses of the mixed salts 1(4+)center dot HP2O73-center dot BF4- and 31(4+)center dot 4H(2)PO(4)(-)center dot 8BF(4)(-) confirmed that receptor 1(4+) can bind the pyrophosphate and phosphate anions in the solid state. C1 [Cai, Jiajia; Yang, Xiaoping; Sessler, Jonathan L.] Univ Texas Austin, Dept Chem & Biochem, Austin, TX 78712 USA. [Hay, Benjamin P.; Young, Neil J.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37830 USA. [Sessler, Jonathan L.] Yonsei Univ, Dept Chem, Seoul 120749, South Korea. RP Hay, BP (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37830 USA. EM haybp@ornl.gov; sessler@cm.utexas.edu FU Office of Basic Energy Sciences, U.S. Department of Energy (DOE) [DE-FG02-01ER15186]; National Science Foundation [CHE-0741973]; Robert A. Welch Foundation [F-1018]; WCU (World Class University) program [R32-2010-000-10217-0]; Ministry of Education, Science and Technology (MEST); Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. DOE FX This work was supported by the Office of Basic Energy Sciences, U.S. Department of Energy (DOE) (grant DE-FG02-01ER15186 to J.L.S.), the National Science Foundation (Grant no. CHE-0741973 for the X-ray diffractometer), and the Robert A. Welch Foundation (F-1018 to J.L.S.). This work was also supported by the WCU (World Class University) program (R32-2010-000-10217-0) administered through the National Research Foundation of Korea funded by the Ministry of Education, Science and Technology (MEST). B.P.H. and N.J.Y. acknowledge support from the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. DOE. NR 77 TC 39 Z9 40 U1 1 U2 64 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2041-6520 J9 CHEM SCI JI Chem. Sci. PY 2013 VL 4 IS 4 BP 1560 EP 1567 DI 10.1039/c3sc22144j PG 8 WC Chemistry, Multidisciplinary SC Chemistry GA 099CV UT WOS:000315597900020 ER PT J AU King, AE Surendranath, Y Piro, NA Bigi, JP Long, JR Chang, CJ AF King, Amanda E. Surendranath, Yogesh Piro, Nicholas A. Bigi, Julian P. Long, Jeffrey R. Chang, Christopher J. TI A mechanistic study of proton reduction catalyzed by a pentapyridine cobalt complex: evidence for involvement of an anation-based pathway SO CHEMICAL SCIENCE LA English DT Article ID ELECTROCATALYTIC HYDROGEN EVOLUTION; MOLYBDENUM-OXO CATALYST; H-2 PRODUCTION; ACTIVE-SITE; LOW OVERPOTENTIALS; DIGLYOXIME CATALYSTS; GENERATING HYDROGEN; AQUEOUS-SOLUTION; WATER REDUCTION; RECENT PROGRESS AB The pentapyridine cobalt complex [Co(PY5Me(2))](2+) and its congeners have been shown to catalyze proton reduction to hydrogen in aqueous solution over a wide pH range using electrical or solar energy input. Here, we employ electrochemical and spectroscopic studies to examine the mechanisms of proton reduction by this parent complex under soluble, diffusion-limited conditions in acetonitrile with acetic acid as the proton donor. Two pathways for proton reduction are identified via cyclic voltammetry: one pathway occurring from an acetonitrile-bound Co-II/I couple and the other pathway operating from an acetate-bound Co-II/I couple. Kinetics studies support protonation of a Co-I species as the rate-determining step for both processes, and additional electrochemical measurements further suggest that the onset of catalysis from the acetonitrile-bound Co-II/I couple is highly affected by catalyst electronics. Taken together, this work not only establishes the CoPY5Me(2) unit as a unique molecular platform that catalyzes the reduction of protons under soluble, diffusion-limited conditions in both aqueous and organic media, but also highlights the participation of anation processes that are likely relevant for a wide range of hydrogen-producing and related catalytic systems. C1 [King, Amanda E.; Surendranath, Yogesh; Piro, Nicholas A.; Bigi, Julian P.; Long, Jeffrey R.; Chang, Christopher J.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Chang, Christopher J.] Univ Calif Berkeley, Dept Mol Biol, Berkeley, CA 94720 USA. [Chang, Christopher J.] Univ Calif Berkeley, Dept Cell Biol, Berkeley, CA 94720 USA. [Chang, Christopher J.] Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA. [Long, Jeffrey R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Piro, Nicholas A.; Bigi, Julian P.; Chang, Christopher J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Long, JR (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM jrlong@berkeley.edu; chrischang@berkeley.edu FU DOE/LBNL grant [403801]; NSF Grant [CHE-1111900]; Miller Institute for Basic Research; National Science Foundation FX This research was funded by DOE/LBNL grant 403801 (C.J.C.). The contributions of J.R.L. were supported by NSF Grant CHE-1111900. C.J.C. is an Investigator with the Howard Hughes Medical Institute. Y.S. and N.A.P. acknowledge the Miller Institute for Basic Research for postdoctoral fellowships, and J.P.B. thanks the National Science Foundation for a graduate fellowship. NR 81 TC 45 Z9 45 U1 2 U2 79 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2041-6520 EI 2041-6539 J9 CHEM SCI JI Chem. Sci. PY 2013 VL 4 IS 4 BP 1578 EP 1587 DI 10.1039/c3sc22239j PG 10 WC Chemistry, Multidisciplinary SC Chemistry GA 099CV UT WOS:000315597900023 ER PT J AU Shreve, AT Elkins, MH Neumark, DM AF Shreve, Alexander T. Elkins, Madeline H. Neumark, Daniel M. TI Photoelectron spectroscopy of solvated electrons in alcohol and acetonitrile microjets SO CHEMICAL SCIENCE LA English DT Article ID HYDRATED ELECTRON; CLUSTER ANIONS; LIQUID WATER; DIELECTRIC PROPERTIES; RADIATION-CHEMISTRY; BINDING-ENERGIES; EXCESS ELECTRONS; BULK WATER; DYNAMICS; METHANOL AB Photoelectron spectra of solvated electrons in methanol, ethanol, and acetonitrile microjets are reported. Solvated electrons are generated in and detached from microjets using two photons from single nanosecond laser pulses at wavelengths ranging 266 to 213 nm. We find vertical binding energies of 3.38 +/- 0.11 eV in methanol and 3.38 +/- 0.10 eV in ethanol. Two features are observed in acetonitrile at 2.61 +/- 0.11 eV and 3.67 +/- 0.15 eV, attributed to the solvated and dimer-bound binding geometries respectively. These results are compared to previous work on solvated cluster anions and alkali-doped solvent clusters. C1 [Shreve, Alexander T.; Elkins, Madeline H.; Neumark, Daniel M.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Shreve, Alexander T.; Neumark, Daniel M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Neumark, DM (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM dneumark@berkeley.edu RI Neumark, Daniel/B-9551-2009 OI Neumark, Daniel/0000-0002-3762-9473 FU National Science Foundation [CHE-1011819] FX Support for this work was provided by the National Science Foundation through Grant CHE-1011819. Thanks to Michael Lipschutz for assistance in preparation of the extra dry acetonitrile solution. NR 78 TC 16 Z9 16 U1 5 U2 71 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2041-6520 J9 CHEM SCI JI Chem. Sci. PY 2013 VL 4 IS 4 BP 1633 EP 1639 DI 10.1039/c3sc22063j PG 7 WC Chemistry, Multidisciplinary SC Chemistry GA 099CV UT WOS:000315597900030 ER PT J AU Li, T Chen, DL Sullivan, JE Kozlowski, MT Johnson, JK Rosi, NL AF Li, Tao Chen, De-Li Sullivan, Jeanne E. Kozlowski, Mark T. Johnson, J. Karl Rosi, Nathaniel L. TI Systematic modulation and enhancement of CO2 : N-2 selectivity and water stability in an isoreticular series of bio-MOF-11 analogues SO CHEMICAL SCIENCE LA English DT Article ID METAL-ORGANIC FRAMEWORK; CARBON-DIOXIDE CAPTURE; INITIO MOLECULAR-DYNAMICS; TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; COORDINATION POLYMER; ADSORPTION PROPERTIES; HIGH-CAPACITY; FORCE-FIELD; SEPARATION AB An isoreticular series of cobalt-adeninate bio-MOFs (bio-MOFs-11-14) is reported. The pores of bio-MOFs-11-14 are decorated with acetate, propionate, butyrate, and valerate, respectively. The nitrogen (N-2) and carbon dioxide (CO2) adsorption properties of these materials are studied and compared. The isosteric heats of adsorption for CO2 are calculated, and the CO2 : N-2 selectivities for each material are determined. As the lengths of the aliphatic chains decorating the pores in bio-MOFs-11-14 increase, the BET surface areas decrease from 1148 m(2) g(-1) to 17 m(2) g(-1) while the CO2 : N-2 selectivities predicted from ideal adsorbed solution theory at 1 bar and 273 K for a 10 : 90 CO2 : N2 mixture range from 73 : 1 for bio-MOF-11 to 123 : 1 for bio-MOF-12 and finally to 107 : 1 for bio-MOF-13. At 298 K, the selectivities are 43 : 1 for bio-MOF-11, 52 : 1 for bio-MOF-12, and 40 : 1 for bio-MOF-13. Additionally, it is shown that bio-MOF-14 exhibits a unique molecular sieving property that allows it to adsorb CO2 but not N2 at 273 and 298 K. Finally, the water stability of bio-MOFs-11-14 increases with increasing aliphatic chain length. Bio-MOF-14 exhibits no loss of crystallinity or porosity after soaking in water for one month. C1 [Li, Tao; Sullivan, Jeanne E.; Kozlowski, Mark T.; Rosi, Nathaniel L.] Univ Pittsburgh, Dept Chem, Pittsburgh, PA 15260 USA. [Chen, De-Li; Johnson, J. Karl] Univ Pittsburgh, Dept Chem & Petr Engn, Pittsburgh, PA 15261 USA. [Johnson, J. Karl] US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. EM nrosi@pitt.edu RI Chen, De-Li/H-6867-2012; Johnson, Karl/E-9733-2013; OI Johnson, Karl/0000-0002-3608-8003; Li, Tao/0000-0001-7586-9841 FU RES [DE-FE0004000]; US DOE [DE-FG02-10ER16164] FX As part of the National Energy Technology Laboratory's Regional University Alliance (NETL-RUA), a collaborative initiative of the NETL, this technical effort was performed under the RES contract DE-FE0004000 (NLR). This work was partially supported by the US DOE through Grant no. DE-FG02-10ER16164 (JKJ). The authors thank Dr Steven Geib, Dr Michael Takase and Dr Allen Oliver for discussion on the crystal structure refinement. The authors also thank the Petersen Institute for Nanoscience and Engineering (PINSE) for access to XRPD instrumentation and the Mechanical Engineering and Materials Science (MEMS) Department for access to SEM instrumentation. NR 53 TC 61 Z9 62 U1 17 U2 178 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2041-6520 J9 CHEM SCI JI Chem. Sci. PY 2013 VL 4 IS 4 BP 1746 EP 1755 DI 10.1039/c3sc22207a PG 10 WC Chemistry, Multidisciplinary SC Chemistry GA 099CV UT WOS:000315597900044 ER PT J AU Martin, RL Haranczyk, M AF Martin, Richard Luis Haranczyk, Maciej TI Exploring frontiers of high surface area metal-organic frameworks SO CHEMICAL SCIENCE LA English DT Article ID CRYSTALLINE POROUS MATERIALS; METHANE STORAGE; ADSORPTION; POROSITY; CAPTURE; DESIGN; TOOLS; NETS AB Metal-organic frameworks (MOFs) have enjoyed considerable interest due to their high internal surface areas as well as tunable pore geometry and chemistry. However, design of optimal MOFs is a great challenge due to the significant number of possible structures. In this work, we present a strategy to rapidly explore the frontiers of these high surface area materials. Here, organic ligands are abstracted by geometrical (alchemical) building blocks, and an optimization of their defining geometrical parameters is performed to identify shapes of ligands which maximize gravimetric surface area of the resulting MOFs. A strength of our approach is that the space of ligands to be explored can be rigorously bounded, allowing discovery of the optimum ligand shape within any criteria, conforming to synthetic requirements or arbitrary exploratory limits. By modifying these bounds, we can project to what extent achievable surface area increases when moving beyond the present limits of organic synthesis. Projecting optimal ligand shapes onto real chemical species, we achieve blueprints for MOFs of various topologies that are predicted to achieve up to 70% higher surface area than the current benchmark materials. C1 [Martin, Richard Luis; Haranczyk, Maciej] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, Berkeley, CA 94720 USA. RP Haranczyk, M (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, Berkeley, CA 94720 USA. EM mharanczyk@lbl.gov RI Haranczyk, Maciej/A-6380-2014; Martin, Richard/C-7129-2013 OI Haranczyk, Maciej/0000-0001-7146-9568; Martin, Richard/0000-0001-9858-2608 FU Laboratory Directed Research and Development Program of the Lawrence Berkeley National Laboratory (LBNL); Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX The authors gratefully acknowledge the input and advice of Yiyi Yao, Jeffrey F. Van Humbeck, Tom M. McDonald, Jeffrey R. Long, David K. Britt and Wendy L. Queen. This work is supported by the Laboratory Directed Research and Development Program of the Lawrence Berkeley National Laboratory (LBNL). LBNL is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DEAC02-05CH11231. NR 31 TC 30 Z9 30 U1 1 U2 42 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2041-6520 J9 CHEM SCI JI Chem. Sci. PY 2013 VL 4 IS 4 BP 1781 EP 1785 DI 10.1039/c3sc00033h PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA 099CV UT WOS:000315597900048 ER PT J AU Liu, PC Zhu, KJ Gao, YF Wu, QL Liu, JS Qiu, JH Gu, QL Zheng, HJ AF Liu, Pengcheng Zhu, Kongjun Gao, Yanfeng Wu, Qingliu Liu, Jinsong Qiu, Jinhao Gu, Qilin Zheng, Hongjuan TI Ultra-long VO2 (A) nanorods using the high-temperature mixing method under hydrothermal conditions: synthesis, evolution and thermochromic properties SO CRYSTENGCOMM LA English DT Article ID PHASE-TRANSITION; INSULATOR-TRANSITION; TRANSFORMATION; MECHANISM; NANOBELTS; POWDERS; OXIDES; FILMS AB Well-crystallized, ultra-long VO2 (A) nanorods were synthesized using a facile high-temperature mixing method (HTMM) under hydrothermal conditions. The as-obtained products were characterized by X-ray diffraction, field-emission scanning electron microscopy, transmission electron microscopy, X-ray photoelectron spectroscopy, UV-Vis-NIR, differential scanning calorimetry and Fourier transform infrared spectroscopy. The effect of W doping on the phase-transition properties of VO2 (A) was also studied. The results indicate that the optimal synthesis condition of VO2 (A) using the HTMM is hydrothermal treatment at 240 degrees C for 48 h with a 3 : 1 molar ratio of the reducing agent to the vanadium source. The reason why the polymorphic forms of VO2 show different colors is that the light in the visible region reflected by the samples is different. The phase-transition temperature of the pure VO2 (A) is 154.75 degrees C, which is significantly lower than the 162 degrees C reported previously. When a small amount of W is doped, VO2 (A) will be transformed into other polymorphic forms, which indicates that the crystal structure of VO2 (A) is highly sensitive to limited doping. Importantly, the as-obtained pure VO2 (A) shows good thermochromic properties and optical-switching characters. A crystal growth mechanism for VO2 (A), oriented-attachment-exfoliation-recrystallization-oriented-attachment, is proposed and described in detail. C1 [Liu, Pengcheng; Zhu, Kongjun; Liu, Jinsong; Qiu, Jinhao; Gu, Qilin; Zheng, Hongjuan] Nanjing Univ Aeronaut & Astronaut, State Key Lab Mech & Control Mech Struct, Nanjing 210016, Peoples R China. [Gao, Yanfeng] Shanghai Univ, Sch Mat Sci & Engn, Baoshan 200444, Peoples R China. [Gao, Yanfeng] Chinese Acad Sci, Shanghai Inst Ceram, State Key Lab High Performance Ceram & Superfine, Shanghai 200050, Peoples R China. [Wu, Qingliu] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Liu, PC (reprint author), Nanjing Univ Aeronaut & Astronaut, State Key Lab Mech & Control Mech Struct, Nanjing 210016, Peoples R China. EM kjzhu@nuaa.edu.cn RI wu, qingliu /C-7631-2012; Gao, Yanfeng/B-3657-2009; Liu (刘), Pengcheng (鹏程)/L-5274-2016; Gu, Qilin/H-6399-2011; OI Liu (刘), Pengcheng (鹏程)/0000-0002-9530-9267; Gu, Qilin/0000-0003-4951-0207; Zhu, Kongjun/0000-0003-0804-8044 FU National Natural Science Foundation of China [51172108, 91023020, 51172265]; Program for Changjiang Scholars and Innovative Research Team in University [IRT0968]; Program for New Century Excellent Talents in University [NCET-10-0070]; Priority Academic Program Development of Jiangsu Higher Education Institutions; National Key Basic Research Project (NKBRP) [2009CB939904]; high-tech project of MOST [2012AA030605, 2012BAA10B03] FX This study was supported by National Natural Science Foundation of China (No. 51172108, No. 91023020, No. 51172265), the Program for Changjiang Scholars and Innovative Research Team in University (IRT0968), the Program for New Century Excellent Talents in University (NCET-10-0070), the Project Funded by the Priority Academic Program Development of Jiangsu Higher Education Institutions, the National Key Basic Research Project (NKBRP, 2009CB939904) and the high-tech project of MOST (2012AA030605, 2012BAA10B03). NR 37 TC 22 Z9 22 U1 7 U2 85 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1466-8033 J9 CRYSTENGCOMM JI Crystengcomm PY 2013 VL 15 IS 14 BP 2753 EP 2760 DI 10.1039/c3ce27085h PG 8 WC Chemistry, Multidisciplinary; Crystallography SC Chemistry; Crystallography GA 104CM UT WOS:000315967200025 ER PT J AU Liu, ZH Qin, L Pang, F Jin, MJ Li, BZ Kang, Y Dale, BE Yuan, YJ AF Liu, Zhi-Hua Qin, Lei Pang, Feng Jin, Ming-Jie Li, Bing-Zhi Kang, Yong Dale, Bruce E. Yuan, Ying-Jin TI Effects of biomass particle size on steam explosion pretreatment performance for improving the enzyme digestibility of corn stover SO INDUSTRIAL CROPS AND PRODUCTS LA English DT Article DE Corn stover; Biomass particle size; Steam explosion pretreatment; Enzymatic hydrolysis; Mass balance ID SACCHAROMYCES-CEREVISIAE 424A(LNH-ST); COMMERCIAL ENZYMES; MOISTURE-CONTENT; LIGNIN REMOVAL; WHEAT-STRAW; CHIP SIZE; HYDROLYSIS; CELLULOSE; TECHNOLOGIES; WOOD AB Size reduction is an essential process for corn stover biomass utilization. Effects of biomass particle size on the efficiency of pretreatment and enzymatic hydrolysis are systematically investigated in the present study. Sugar recoveries and conversions of the biomass with particle sizes at 2.5, 2.0, 1.5, 1.0 and 0.5 cm were compared. The highest sugar recovery reached 99.6% for glucan and 67.0% for xylan at the particle size of 1.0 and 0.5 cm, respectively, but the highest sugar conversion (100% for glucan and 83% for xylan) was observed at the particle size of 2.5 cm. The enzymatic hydrolysis rate and conversion of pretreated biomass obviously increased with increasing biomass particle size. With increase of biomass particle size, the specific surface area of pretreated biomass significantly increased and the crystallinity index of pretreated biomass apparently decreased. In studied extent of particle sizes, the utilization of larger biomass particles would be desirable to achieve the high pretreatment efficiency and hence improve subsequent enzymatic hydrolysis performance compared with the smaller ones. (C) 2012 Elsevier B.V. All rights reserved. C1 [Liu, Zhi-Hua; Qin, Lei; Li, Bing-Zhi; Yuan, Ying-Jin] Tianjin Univ, Sch Chem Engn & Technol, Dept Pharmaceut Engn, Minist Educ,Key Lab Syst Bioengn, Tianjin 300072, Peoples R China. [Pang, Feng; Kang, Yong] Tianjin Univ, Sch Chem Engn & Technol, Tianjin 300072, Peoples R China. [Jin, Ming-Jie; Dale, Bruce E.] Michigan State Univ, US DOE, Great Lakes Bioenergy Res Ctr, Lansing, MI USA. [Jin, Ming-Jie; Dale, Bruce E.] Michigan State Univ, Dept Chem Engn & Mat Sci, Biomass Convers Res Lab, Lansing, MI 48910 USA. RP Li, BZ (reprint author), Tianjin Univ, Sch Chem Engn & Technol, Dept Pharmaceut Engn, Minist Educ,Key Lab Syst Bioengn, POB 6888, Tianjin 300072, Peoples R China. EM bzli@tju.edu.cn RI Li, Bing-Zhi/I-6107-2013; OI Li, Bing-Zhi/0000-0003-4121-3048; Jin, Mingjie/0000-0002-9493-305X FU National Basic Research Program of China ("973" Program) [2013CB733600]; National Natural Science Foundation of China [21020102040]; National High Technology Research and Development Program ("863" Program) [2012AA02A701] FX This work was funded by the National Basic Research Program of China ("973" Program: 2013CB733600), the National Natural Science Foundation of China (Major International Joint Research Project: 21020102040), and the National High Technology Research and Development Program ("863" Program: 2012AA02A701). We thank Genecor International Corporation (Suzhou, China) for kindly providing the enzymes. NR 36 TC 47 Z9 49 U1 4 U2 70 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0926-6690 J9 IND CROP PROD JI Ind. Crop. Prod. PD JAN PY 2013 VL 44 BP 176 EP 184 DI 10.1016/j.indcrop.2012.11.009 PG 9 WC Agricultural Engineering; Agronomy SC Agriculture GA 099XO UT WOS:000315659400027 ER PT J AU Cook, AW Ulitsky, MS Miller, DS AF Cook, Andrew W. Ulitsky, Mark S. Miller, Douglas S. TI Hyperviscosity for unstructured ALE meshes SO INTERNATIONAL JOURNAL OF COMPUTATIONAL FLUID DYNAMICS LA English DT Article DE artificial viscosity; ALE; unstructured grid; shocks; turbulence; vorticity ID LARGE-EDDY SIMULATIONS; ARTIFICIAL VISCOSITY; NUMERICAL-METHODS; REACTING FLOWS; TURBULENCE; CONSERVATION; ALGORITHM; NUMBER; ENERGY; SHOCKS AB An artificial viscosity, originally designed for Eulerian schemes, is adapted for use in arbitrary LagrangianEulerian simulations. Changes to the Eulerian model (dubbed hyperviscosity') are discussed, which enable it to work within a Lagrangian framework. New features include a velocity-weighted grid scale and a generalised filtering procedure, applicable to either structured or unstructured grids. The model employs an artificial shear viscosity for treating small-scale vorticity and an artificial bulk viscosity for shock capturing. The model is based on the NavierStokes form of the viscous stress tensor, including the diagonal rate-of-expansion tensor. A second-order version of the model is presented, in which Laplacian operators act on the velocity divergence and the grid-weighted strain-rate magnitude to ensure that the velocity field remains smooth at the grid scale. Unlike sound-speed-based artificial viscosities, the hyperviscosity model is compatible with the low Mach number limit. The new model outperforms a commonly used Lagrangian artificial viscosity on a variety of test problems. C1 [Cook, Andrew W.; Ulitsky, Mark S.; Miller, Douglas S.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Cook, AW (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM awcook@llnl.gov FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract no. DE-AC52-07NA27344. NR 50 TC 5 Z9 5 U1 1 U2 11 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND SN 1061-8562 J9 INT J COMPUT FLUID D JI Int. J. Comput. Fluid Dyn. PD JAN 1 PY 2013 VL 27 IS 1 BP 32 EP 50 DI 10.1080/10618562.2012.756477 PG 19 WC Mechanics; Physics, Fluids & Plasmas SC Mechanics; Physics GA 101ML UT WOS:000315779000003 ER PT J AU Aad, G Abajyan, T Abbott, B Abdallah, J Khalek, SA Abdelalim, AA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Acharya, BS Adamczyk, L Adams, DL Addy, TN Adelman, J Adomeit, S Adragna, P Adye, T Aefsky, S Aguilar-Saavedra, JA Agustoni, M Aharrouche, M Ahlen, SP Ahles, F Ahmad, A Ahsan, M Aielli, G Akesson, TPA Akimoto, G Akimov, AV Alam, MS Alam, MA Albert, J Albrand, S Aleksa, M Aleksandrov, IN Alessandria, F Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Aliev, M Alimonti, G Alison, J Allbrooke, BMM Allport, PP Allwood-Spiers, SE Almond, J Aloisio, A Alon, R Alonso, A Alonso, F Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Amelung, C Ammosov, VV Dos Santos, SPA Amorim, A Amram, N Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Andrieux, ML Anduaga, XS Angelidakis, S Anger, P Angerami, A Anghinolfi, F Anisenkov, A Anjos, N Annovi, A Antonaki, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Aoun, S Bella, LA Apolle, R Arabidze, G Aracena, I Arai, Y Arce, ATH Arfaoui, S Arguin, JF Argyropoulos, S Arik, E Arik, M Armbruster, AJ Arnaez, O Arnal, V Arnault, C Artamonov, A Artoni, G Arutinov, D Asai, S Ask, S Asman, B Asquith, L Assamagan, K Astbury, A Atkinson, M Aubert, B Auge, E Augsten, K Aurousseau, M Avolio, G Avramidou, R Axen, D Azuelos, G Azuma, Y Baak, MA Baccaglioni, G Bacci, C Bach, AM Bachacou, H Bachas, K Backes, M Backhaus, M Mayes, JB Badescu, E Bagnaia, P Bahinipati, S Bai, Y Bailey, DC Bain, T Baines, JT Baker, OK Baker, MD Baker, S Balek, P Banas, E Banerjee, P Banerjee, S Banfi, D Bangert, A Bansal, V Bansil, HS Barak, L Baranov, SP Galtieri, AB Barber, T Barberio, EL Barberis, D Barbero, M Bardin, DY Barillari, T Barisonzi, M Barklow, T Barlow, N Barnett, BM Barnett, 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Zmouchko, V. V. Zobernig, G. Zoccoli, A. zur Nedden, M. Zutshi, V. Zwalinski, L. CA ATLAS Collaboration TI Search for resonances decaying into top-quark pairs using fully hadronic decays in pp collisions with ATLAS at root s=7 TeV SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering ID FORWARD-BACKWARD ASYMMETRY; P(P)OVER-BAR COLLISIONS; T(T)OVER-BAR AB A search for resonances produced in 7 TeV proton-proton collisions and decaying into top-quark pairs is described. In this Letter events where the top-quark decay produces two massive jets with large transverse momenta recorded with the ATLAS detector at the Large Hadron Collider are considered. Two techniques that rely on jet substructure are used to separate top-quark jets from those arising from light quarks and gluons. In addition, each massive jet is required to have evidence of an associated bottom-quark decay. 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L.] Univ Sao Paulo, Inst Fis, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Baker, M. D.; Begel, M.; Bernius, C.; Chen, H.; Chernyatin, V.; Debbe, R.; Dhullipudi, R.; Ernst, M.; Gadfort, T.; Gibbard, B.; Gordon, H. A.; Greenwood, Z. D.; Klimentov, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Majewski, S.; Metcalfe, J.; Nevski, P.; Okawa, H.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Park, W.; Pleier, M. -A.; Poblaguev, A.; Polychronakos, V.; Pravahan, R.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rahm, D.; Rajagopalan, S.; Redlinger, G.; Sawyer, L.; Sircar, A.; Snyder, S.; Steinberg, P.; Stumer, I.; Subramaniam, R.; Takai, H.; Tamsett, M. C.; Triplett, N.; Undrus, A.; Wenaus, T.; Ye, S.; Yu, D.; Zaytsev, A.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Badescu, E.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Cuciuc, C. -M.; Dinut, F.; Dita, P.; Dita, S.; Micu, L.; Olariu, A.; Pantea, D.; Popeneciu, G. A.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Darlea, G. L.] Univ Politeh Bucharest, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Gonzalez Silva, M. L.; Otero y Garzon, G.; Piegaia, R.; Romeo, G.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Ask, S.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Buttinger, W.; Carter, J. R.; Chapman, J. D.; Cowden, C.; French, S. T.; Frost, J. A.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Moeller, V.; Parker, M. A.; Robinson, D.; Sandoval, T.; Thomson, M.; Ward, C. P.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Gillberg, D.; Koffas, T.; Lacey, J.; Liu, C.; Marchand, J. F.; McCarthy, T. G.; Oakham, F. G.; Randrianarivony, K.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Anastopoulos, C.; Anghinolfi, F.; Avolio, G.; Baak, M. A.; Bachas, K.; Banfi, D.; Battistin, M.; Bellomo, M.; Beltramello, O.; Berge, D.; Bianchi, R. M.; Blanchot, G.; Bogaerts, J. A.; Boyd, J.; Bremer, J.; Burckhart, H.; Byszewski, M.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Catmore, J. R.; Cattai, A.; Cerri, A.; Barajas, C. A. Chavez; Childers, J. T.; Chromek-Burckhart, D.; Cote, D.; Danielsson, H. O.; Dell'Acqua, A.; Di Girolamo, A.; Di Girolamo, B.; Di Micco, B.; Dittus, F.; Dobos, D.; Dobson, E.; Dopke, J.; Dudarev, A.; Duehrssen, M.; Ellis, N.; Elsing, M.; Fabre, C.; Farthouat, P.; Fassnacht, P.; Francis, D.; Franz, S.; Froeschl, R.; Froidevaux, D.; Torregrosa, E. Fullana; Gabaldon, C.; Garelli, N.; Garonne, V.; Gianotti, F.; Gibson, S. M.; Godlewski, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Haas, S.; Hahn, F.; Hauschild, M.; Hawkings, R. J.; Heller, M.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Huhtinen, M.; Jaekel, M. R.; Jansen, H.; Jenni, P.; Joram, C.; Jungst, R. M.; Kaneda, M.; Kaplon, J.; Kerschen, N.; Klioutchnikova, T.; Koeneke, K.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malaescu, B.; Malyukov, S.; Mapelli, A.; Mapelli, L.; Marshall, Z.; Martin, B.; Messina, A.; Michal, S.; Molfetas, A.; Morley, A. K.; Mornacchi, G.; Muenstermann, D.; Nairz, A. M.; Nakahama, Y.; Negri, G.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Ohm, C. C.; Palestini, S.; Pauly, T.; Perez, G.; Pernegger, H.; Peters, K.; Petersen, B. A.; Petersen, J.; Piacquadio, G.; Pommes, K.; Poppleton, A.; Bueso, X. Portell; Poulard, G.; Prasad, S.; Raymond, M.; Rembser, C.; Dos Santos, D. Roda; Roe, S.; Salek, D.; Salzburger, A.; Savu, D. O.; Schlenker, S.; Schott, M.; Sfyrla, A.; Spigo, G.; Spiwoks, R.; Stewart, G. A.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van der Ster, D.; van Eldik, N.; Vandelli, W.; Veness, R.; Vinek, E.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Winklmeier, F.; Wotschack, J.; Zajacova, Z.; Zwalinski, L.] CERN, Geneva, Switzerland. [Anderson, K. J.; Boveia, A.; Canelli, F.; Cheng, Y.; Choudalakis, G.; Fiascaris, M.; Gardner, R. W.; Plante, I. Jen-La; Kapliy, A.; Li, H. L.; Meehan, S.; Melachrinos, C.; Merritt, F. S.; Meyer, C.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Shochet, M. J.; Tompkins, L.; Tuggle, J. M.; Vukotic, I.; Webster, J. S.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Diaz, M. A.; Olivares Pino, S. A.; Quinonez, F.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Carquin, E.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lu, F.; Ouyang, Q.; Ruan, X.; Shan, L. Y.; Wang, J.; Yao, L.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Han, L.; Jiang, Y.; Li, B.; Li, S.; Liu, M.; Liu, Y.; Peng, H.; Wu, Y.; Xu, C.; Xu, L.; Zhang, D.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Feng, C.; Ge, P.; Meng, Z.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200030, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Toro, R. Camacho; Cinca, D.; Donini, J.; Febbraro, R.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Vazeille, F.] Univ Clermont Ferrand, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Toro, R. Camacho; Cinca, D.; Donini, J.; Febbraro, R.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Toro, R. Camacho; Cinca, D.; Donini, J.; Febbraro, R.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Vazeille, F.] Univ Clermont Ferrand, Photochim Mol & Macromol Lab, CNRS, IN2P3, F-63177 Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Brooijmans, G.; Chen, Y.; Dodd, J.; Grau, N.; Guo, J.; Hu, D.; Hughes, E. W.; Nikiforou, N.; Parsons, J. A.; Penson, A.; Perez, K.; Reale, V. Perez; Scherzer, M. I.; Spousta, M.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Williams, E.; Willis, W.; Wulf, E.; Zivkovic, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Boelaert, N.; Dam, M.; Gregersen, K.; Hansen, J. R.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Heisterkamp, S.; Jakobsen, S.; Loevschall-Jensen, A. E.; Jez, P.; Joergensen, M. D.; Kadlecik, P.; Klinkby, E. B.; Lundquist, J.; Mackeprang, R.; Mehlhase, S.; Petersen, T. C.; Simonyan, M.; Thomsen, L. A.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; Fazio, S.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Morello, G.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] INFN Grp Collegato Cosenza, Milan, Italy. [Capua, M.; Crosetti, G.; Fazio, S.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Morello, G.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Banas, E.; Blocki, J.; de Renstrom, P. A. Bruckman; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Malecki, P.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Turala, M.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.; Zemla, A.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Yagci, K. Dindar; Firan, A.; Hoffman, J.; Joffe, D.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Rios, R. R.; Sekula, S. J.; Stroynowski, R.; Wang, H.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Ahsan, M.; Izen, J. M.; Lou, X.; Reeves, K.; Wong, W. C.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Kuutmann, E. Bergeaas; Bloch, I.; Dassoulas, J. A.; Dietrich, J.; Ehrenfeld, W.; Ferrara, V.; Fischer, G.; Friedrich, C.; Glazov, A.; Goebel, M.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K-J.; Gregor, I. M.; Hiller, K. H.; Huettmann, A.; Belenguer, M. Jimenez; Johnert, S.; Karnevskiy, M.; Katzy, J.; Kono, T.; Kuhl, T.; Lange, C.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Cavalcanti, T. Perez; Petschull, D.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Zhu, H.] DESY, Hamburg, Germany. [Argyropoulos, S.; Kuutmann, E. Bergeaas; Bloch, I.; Dassoulas, J. A.; Dietrich, J.; Ehrenfeld, W.; Ferrara, V.; Fischer, G.; Friedrich, C.; Glazov, A.; Goebel, M.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K-J.; Gregor, I. M.; Hiller, K. H.; Huettmann, A.; Belenguer, M. Jimenez; Johnert, S.; Karnevskiy, M.; Katzy, J.; Kono, T.; Kuhl, T.; Lange, C.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Cavalcanti, T. Perez; Petschull, D.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Zhu, H.] DESY, Zeuthen, Germany. [Bunse, M.; Esch, H.; Goessling, C.; Hirsch, F.; Jung, C. A.; Klingenberg, R.; Reisinger, I.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Czodrowski, P.; Friedrich, F.; Goepfert, T.; Kobel, M.; Leonhardt, K.; Ludwig, A.; Mader, W. F.; Morgenstern, M.; Rudolph, C.; Schnoor, U.; Schwierz, R.; Seifert, F.; Steinbach, P.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Ebenstein, W. L.; Fowler, A. J.; Ko, B. R.; Kotwal, A.; Kruse, M. K.; Oh, S. H.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Buckley, A. G.; Clark, P. J.; Debenedetti, C.; Harrington, R. D.; Martin, V. J.; O'Brien, B. J.; Schaelicke, A.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Cerutti, F.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.; Volpi, G.] INFN Lab Nazl Frascati, Frascati, Italy. [Aad, G.; Ahles, F.; Barber, T.; Bernhard, R.; Boehler, M.; Bruneliere, R.; Christov, A.; Consorti, V.; Fehling-Kaschek, M.; Flechl, M.; Hartert, J.; Herten, G.; Horner, S.; Jakobs, K.; Janus, M.; Kononov, A. I.; Kuehn, S.; Lai, S.; Landgraf, U.; Lohwasser, K.; Ludwig, I.; Ludwig, J.; Mahboubi, K.; Mohr, W.; Nilsen, H.; Parzefall, U.; Rammensee, M.; Rave, T. C.; Rurikova, Z.; Schmidt, E.; Schumacher, M.; Siegert, F.; Stoerig, K.; Sundermann, J. E.; Temming, K. K.; Thoma, S.; Tsiskaridze, V.; Venturi, M.; Vivarelli, I.; von Radziewski, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Winkelmann, S.; Xie, S.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Abdelalim, A. A.; Alexandre, G.; Backes, M.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; Blondel, A.; Bucci, F.; Clark, A.; Dao, V.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Iacobucci, G.; La Rosa, A.; Lister, A.; Latour, B. Martin dit; Mermod, P.; Herrera, C. Mora; Nektarijevic, S.; Nessi, M.; Nikolics, K.; Pasztor, G.; Picazio, A.; Pohl, M.; Rosbach, K.; Rosselet, L.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Beccherle, R.; Caso, C.; Dameri, M.; Darbo, G.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] INFN Sez Genova, Genoa, Italy. [Barberis, D.; Caso, C.; Dameri, M.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Chikovani, L.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Khubua, J.; Mchedlidze, G.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Bussey, P.; Buttar, C. M.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Edwards, N. C.; Ferrag, S.; Ferrando, J.; De Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Kar, D.; Kenyon, M.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Robson, A.; Saxon, D. H.; Smith, K. M.; Denis, R. D. St.; Steele, G.; Thompson, A. S.; Wraight, K.; Wright, M.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bierwagen, K.; Blumenschein, U.; Brandt, O.; Erdmann, J.; Evangelakou, D.; George, M.; Grosse-Knetter, J.; Guindon, S.; Hamer, M.; Hensel, C.; Keil, M.; Knue, A.; Kohn, F.; Krieger, N.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Mann, A.; Meyer, J.; Morel, J.; Nackenhorst, O.; Pashapour, S.; Quadt, A.; Roe, A.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Uhrmacher, M.; Schroeder, T. Vazquez; Weingarten, J.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Andrieux, M-L.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Stark, J.; Sun, X.; Weydert, C.] Univ Grenoble 1, Lab Phys Subatom & Cosmol, Grenoble, France. [Albrand, S.; Andrieux, M-L.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Stark, J.; Sun, X.; Weydert, C.] CNRS, IN2P3, Grenoble, France. [Albrand, S.; Andrieux, M-L.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Stark, J.; Sun, X.; Weydert, C.] Inst Natl Polytech Grenoble, F-38031 Grenoble, France. [Addy, T. N.; Harvey, A.; McFarlane, K. W.; Shin, T.; Vassilakopoulos, V. I.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Belloni, A.; Catastini, P.; Conti, G.; Franklin, M.; Huth, J.; Jeanty, L.; Kagan, M.; Mateos, D. Lopez; Outschoorn, V. Martinez; Mercurio, K. M.; Mills, C.; Morii, M.; Skottowe, H. P.; Smith, B. C.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Anders, G.; Andrei, V.; Davygora, Y.; Dietzsch, T. A.; Dunford, M.; Geweniger, C.; Hanke, P.; Henke, M.; Khomich, A.; Kluge, E. -E.; Lang, V. S.; Lendermann, V.; Lepold, F.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Kugel, A.; Maenner, R.; Schroer, N.] Heidelberg Univ, ZITI Inst Tech Informat, Heidelberg, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Cwetanski, P.; Evans, H.; Gagnon, P.; Jain, V.; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Price, D.; Whittington, D.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Epp, B.; Jussel, P.; Kneringer, E.; Kuhn, D.; Lukas, W.; Rudolph, G.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Behera, P. K.; Limper, M.; Mallik, U.; Pylypchenko, Y.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Rosenberg, E. I.; Ruiz-Martinez, A.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Aleksandrov, I. N.; Bardin, D. Y.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Grigalashvili, N.; Huseynov, N.; Kalinovskaya, L. V.; Kazarinov, M. Y.; Kekelidze, G. D.; Kharchenko, D.; Khramov, E.; Kolesnikov, V.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Pozdnyakov, V.; Rumyantsev, L.; Rusakovich, N. A.; Sadykov, R.; Shiyakova, M.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.; Zimin, N. I.] Joint Inst Nucl Res Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Arai, Y.; Doi, Y.; Haruyama, T.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Makida, Y.; Manabe, A.; Mitsui, S.; Nagano, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Trocme, B.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Hayakawa, T.; King, M.; Kishimoto, T.; Kitamura, T.; Kurashige, H.; Matsushita, T.; Ochi, A.; Suzuki, Y.; Takeda, H.; Tani, K.; Watanabe, I.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Sasao, N.; Sumida, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Davidson, R.; de Mora, L.; Dearnaley, W. J.; Fox, H.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Bianco, M.; Cataldi, G.; Chiodini, G.; Gorini, E.; Grancagnolo, F.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] INFN Sez Lecce, Lecce, Italy. [Bianco, M.; Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Greenshaw, T.; Gwilliam, C. B.; Hayward, H. S.; Jackson, J. N.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kluge, T.; Kretzschmar, J.; Laycock, P.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Sellers, G.; Vossebeld, J. H.; Waller, P.; Wrona, B.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Dolenc, I.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Dolenc, I.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia. [Adragna, P.; Bona, M.; Carter, A. A.; Cerrito, L.; Eisenhandler, E.; Ellis, K.; Goddard, J. R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Poll, J.; Rizvi, E.; Salamanna, G.; Castanheira, M. Teixeira Dias; Wiglesworth, C.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Alam, M. A.; Berry, T.; Boisvert, V.; Brooks, T.; Cantrill, R.; Cowan, G.; Duguid, L.; Edwards, C. A.; George, S.; Goncalo, R.; Hayden, D.; Vazquez, J. G. Panduro; Pastore, Fr.; Rose, M.; Spano, F.; Strong, J. A.; Teixeira-Dias, P.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Baker, S.; Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Chislett, R. T.; Christidi, I. A.; Cooper, B. D.; Davison, A. R.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Lambourne, L.; Monk, J.; Nash, M.; Nurse, E.; Prabhu, R.; Sherwood, P.; Simmons, B.; Taylor, C.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Cavalleri, P.; Chareyre, E.; Crescioli, F.; Davignon, O.; De Cecco, S.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph.; Theveneaux-Pelzer, T.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Cavalleri, P.; Chareyre, E.; Crescioli, F.; Davignon, O.; De Cecco, S.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph.; Theveneaux-Pelzer, T.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Cavalleri, P.; Chareyre, E.; Crescioli, F.; Davignon, O.; De Cecco, S.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph.; Theveneaux-Pelzer, T.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Alonso, A.; Bocchetta, S. S.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Jarlskog, G.; Lundberg, B.; Lytken, E.; Meirose, B.; Mjornmark, J. U.; Smirnova, O.] Lund Univ, Fysiska Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Labarga, L.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Aharrouche, M.; Arnaez, O.; Blum, W.; Buescher, V.; Caputo, R.; Eckweiler, S.; Edmonds, K.; Ellinghaus, F.; Ertel, E.; Fiedler, F.; Fleckner, J.; Goeringer, C.; Handel, C.; Hohlfeld, M.; Hsu, P. J.; Ji, W.; Kawamura, G.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lungwitz, M.; Masetti, L.; Meyer, C.; Moreno, D.; Mueller, T.; Neusiedl, A.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schroeder, C.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Almond, J.; Borri, M.; Brown, G.; Chavda, V.; Cox, B. E.; Da Via, C.; Duerdoth, I. P.; Forti, A.; Howarth, J.; Ibbotson, M.; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Marx, M.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Pilkington, A. D.; Robinson, J. E. M.; Schwanenberger, C.; Snow, S. W.; Watts, S.; Woudstra, M. J.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aoun, S.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Li, S.; Maurer, J.; Monnier, E.; Odier, J.; Pralavorio, P.; Rozanov, A.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aoun, S.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Li, S.; Maurer, J.; Monnier, E.; Odier, J.; Pralavorio, P.; Rozanov, A.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Brau, B.; Colon, G.; Dallapiccola, C.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Caron, B.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Dobbs, M.; Dufour, M-A.; Klemetti, M.; Mc Donald, J.; Robertson, S. H.; Rios, C. Santamarina; Schram, M.; Stockton, M. C.; Vachon, B.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Davidson, N.; Diglio, S.; Hamano, K.; Jennens, D.; Kubota, T.; Limosani, A.; Moorhead, G. F.; Hanninger, G. Nunes; Phan, A.; Shao, Q. T.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Volpi, M.; White, M. J.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Armbruster, A. J.; Borroni, S.; Chapman, J. W.; Cirilli, M.; Dai, T.; Diehl, E. B.; Ferretti, C.; Goldfarb, S.; Harper, D.; Levin, D.; Li, X.; Liu, H.; Liu, J. B.; Liu, L.; Mc Kee, S. P.; Neal, H. A.; Panikashvili, N.; Purdham, J.; Qian, J.; Scheirich, D.; Thun, R. P.; Walch, S.; Wilson, A.; Wooden, G.; Wu, Y.; Yang, H.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Fedorko, W.; Hauser, R.; Holzbauer, J. L.; Huston, J.; Koll, J.; Linnemann, J. T.; Martin, B.; Miller, R. J.; Pope, B. G.; Schwienhorst, R.; Stelzer, H. J.; Tollefson, K.; True, P.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alessandria, F.; Alimonti, G.; Andreazza, A.; Baccaglioni, G.; Besana, M. I.; Broggi, F.; Carminati, L.; Cavalli, D.; Citterio, M.; Consonni, S. M.; Costa, G.; Fanti, M.; Favareto, A.; Giugni, D.; Koletsou, I.; Lari, T.; Mandelli, L.; Mazzanti, M.; Meloni, F.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Rivoltella, G.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Vegni, G.; Volpini, G.] INFN Sez Milano, Milan, Italy. [Andreazza, A.; Besana, M. I.; Carminati, L.; Consonni, S. M.; Fanti, M.; Favareto, A.; Meloni, F.; Perini, L.; Pizio, C.; Ragusa, F.; Rivoltella, G.; Simoniello, R.; Turra, R.; Vegni, G.] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Satsounkevitch, I.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus. [Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Banerjee, P.; Bouchami, J.; Davies, M.; Giunta, M.; Leroy, C.; Martin, J. P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.] Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.] Moscow Engn & Phys Inst MEPhI, Moscow, Russia. [Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Beale, S.; Becker, S.; Biebel, O.; Bortfeldt, J.; Calfayan, P.; de Graat, J.; Duckeck, G.; Ebke, J.; Elmsheuser, J.; Engl, A.; Galea, C.; Heller, C.; Hertenberger, R.; Kummer, C.; Legger, F.; Lichtnecker, M.; Lorenz, J.; Mameghani, R.; Mueller, T. A.; Nunnemann, T.; Oakes, L. B.; Rauscher, F.; Reznicek, P.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Schieck, J.; Serfon, C.; Staude, A.; Vladoiu, D.; Walker, R.; Will, J. Z.; Zhuang, X.; Zibell, A.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Beimforde, M.; Bethke, S.; Bittner, B.; Bronner, J.; Capriotti, D.; Compostella, G.; Cortiana, G.; Dubbert, J.; Flowerdew, M. J.; Giovannini, P.; Ince, T.; Jantsch, A.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kotov, S.; Kroha, H.; Macchiolo, A.; Manfredini, A.; Menke, S.; Moser, H. G.; Nagel, M.; Nisius, R.; Oberlack, H.; Pahl, C.; Pospelov, G. E.; Potrap, I. N.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Stern, S.; Stonjek, S.; Vanadia, M.; von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.; Zhuravlov, V.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Shimizu, S.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Shimizu, S.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Capasso, L.; Carlino, G.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; della Volpe, D.; Di Donato, C.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Patricelli, S.; Sanchez, A.; Sekhniaidze, G.] INFN Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Capasso, L.; Chiefari, G.; della Volpe, D.; Di Donato, C.; Giordano, R.; Merola, L.; Patricelli, S.; Sanchez, A.] Univ Naples Federico II, Dipartimento Sci Fisiche, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Chelstowska, M. A.; De Groot, N.; Filthaut, F.; Klok, P. F.; Konig, A. C.; Koetsveld, F.; Raas, M.; Salvucci, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Doxiadis, A. D.; Ferrari, P.; Garitaonandia, H.; Geerts, D. A. A.; Gosselink, M.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kayl, M. S.; Klous, S.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Luijckx, G.; Mahlstedt, J.; Massaro, G.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Pani, P.; Rijpstra, M.; Ruckstuhl, N.; Ta, D.; Tsiakiris, M.; Turlay, E.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van der Poel, E.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.] Nikhef Natl Inst Subatom Phys, Amsterdam, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Doxiadis, A. D.; Ferrari, P.; Garitaonandia, H.; Geerts, D. A. A.; Gosselink, M.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kayl, M. S.; Klous, S.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Luijckx, G.; Mahlstedt, J.; Massaro, G.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Pani, P.; Rijpstra, M.; Ruckstuhl, N.; Ta, D.; Tsiakiris, M.; Turlay, E.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van der Poel, E.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.] Univ Amsterdam, Amsterdam, Netherlands. [Calkins, R.; Chakraborty, D.; Cole, S.; de Lima, J. G. Rocha; Suhr, C.; Yurkewicz, A.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL USA. [Anisenkov, A.; Beloborodova, O.; Bobrovnikov, V. S.; Bogdanchikov, A.; Kazanin, V. F.; Kolachev, G. M.; Korol, A.; Malyshev, V.; Maslennikov, A. L.; Maximov, D. A.; Orlov, I.; Peleganchuk, S. V.; Schamov, A. G.; Skovpen, K.; Soukharev, A.; Talyshev, A.; Tikhonov, Y. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Budick, B.; Casadei, D.; Cranmer, K.; Haas, A.; van Huysduynen, L. Hooft; Kaplan, B.; Konoplich, R.; Krasznahorkay, A.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.; Prokofiev, K.; Zhao, L.] NYU, Dept Phys, New York, NY 10003 USA. [Fisher, M. J.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Rahimi, A. M.; Strang, M.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Gutierrez, P.; Jana, D. K.; Marzin, A.; Meera-Lebbai, R.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Snow, J.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Khanov, A.; Rizatdinova, F.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Hamal, P.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Potter, C. T.; Ptacek, E.; Radloff, P.; Reinsch, A.; Searcy, J.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Andari, N.; Arnault, C.; Auge, E.; Barrillon, P.; Benoit, M.; Binet, S.; Bourdarios, C.; De La Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Matricon, P.; Niedercorn, F.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Ruan, X.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Teinturier, M.; Veillet, J. J.; Wicek, F.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Andari, N.; Arnault, C.; Auge, E.; Barrillon, P.; Benoit, M.; Binet, S.; Bourdarios, C.; De La Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Matricon, P.; Niedercorn, F.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Ruan, X.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Teinturier, M.; Veillet, J. J.; Wicek, F.; Zerwas, D.; Zhang, Z.] CNRS, IN2P3, F-91405 Orsay, France. [Hanagaki, K.; Hirose, M.; Lee, J. S. H.; Meguro, T.; Nomachi, M.; Okamura, W.; Sugaya, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Buran, T.; Cameron, D.; Gjelsten, B. K.; Gramstad, E.; Lund, E.; Ould-Saada, F.; Pajchel, K.; Read, A. L.; Rohne, O.; Samset, B. H.; Smestad, L.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Apolle, R.; Barr, A. J.; Boddy, C. R.; Brandt, G.; Buchanan, J.; Buckingham, R. M.; Cooper-Sarkar, A. M.; Dafinca, A.; Davies, E.; Gallas, E. J.; Gwenlan, C.; Hall, D.; Hays, C. P.; Howard, J.; Huffman, T. B.; Issever, C.; King, R. S. B.; Kogan, L. A.; Korn, A.; Larner, A.; Lewis, A.; Liang, Z.; Livermore, S. S. A.; Mattravers, C.; Nickerson, R. B.; Pinder, A.; Robichaud-Veronneau, A.; Ryder, N. C.; Short, D.; Tseng, J. C-L.; Vickey, T.; Viehhauser, G. H. A.; Weidberg, A. R.; Whitehead, S. R.; Young, C. J.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Colombo, T.; Conta, C.; Ferrari, R.; Franchino, S.; Fraternali, M.; Gaudio, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Uslenghi, M.; Vercesi, V.] INFN Sez Pavia, Pavia, Italy. [Colombo, T.; Conta, C.; Franchino, S.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.; Uslenghi, M.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Alison, J.; Brendlinger, K.; Degenhardt, J.; Dressnandt, N.; Fratina, S.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Keener, P. T.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Newcomer, F. M.; Olivito, D.; Ospanov, R.; Reece, R.; Saxon, J.; Schaefer, D.; Stahlman, J.; Thomson, E.; Van Berg, R.; Wagner, P.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Bertolucci, F.; Cascella, M.; Cavasinni, V.; Del Prete, T.; Dotti, A.; Roda, C.; Sarri, F.; White, S.; Zinonos, Z.] INFN Sez Pisa, Pisa, Italy. [Bertolucci, F.; Cascella, M.; Cavasinni, V.; Del Prete, T.; Dotti, A.; Roda, C.; Sarri, F.; White, S.; Zinonos, Z.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Boudreau, J.; Cleland, W.; Escobar, C.; Kittelmann, T.; Mueller, J.; Prieur, D.; Savinov, V.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Anjos, N.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Wemans, A. Do Valle; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Jorge, P. M.; Lopes, L.; Machado Miguens, J.; Maio, A.; Maneira, J.; Oliveira, M.; Onofre, A.; Palma, A.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. [Bohm, J.; Chudoba, J.; Gallus, P.; Gunther, J.; Jakoubek, T.; Juranek, V.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Marcisovsky, M.; Mikestikova, M.; Myska, M.; Nemecek, S.; Ruzicka, P.; Schovancova, J.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Tic, T.; Valenta, J.; Vrba, V.; Zeman, M.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Balek, P.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Kodys, P.; Leitner, R.; Novakova, J.; Rybar, M.; Spousta, M.; Strachota, P.; Suk, M.; Sykora, T.; Tas, P.; Valkar, S.; Vorobel, V.; Wilhelm, I.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Augsten, K.; Holy, T.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Kral, V.; Krejci, F.; Pospisil, S.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solar, M.; Solc, J.; Sopko, V.; Sopko, B.; Stekl, I.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.] Czech Tech Univ, Prague, Czech Republic. [Ammosov, V. V.; Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Ivashin, A. V.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.; Zmouchko, V. V.] State Res Ctr Inst High Energy Phys, Protvino, Russia. [Adye, T.; Apolle, R.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Gillman, A. R.; Haywood, S. J.; Kirk, J.; Mattravers, C.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Nash, M.; Norton, P. R.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Benslama, K.; Smit, G. V. Ybeles] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Artoni, G.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Pedis, D.; De Salvo, A.; De Zorzi, G.; Dionisi, C.; Falciano, S.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Rossi, E.; Tehrani, F. Safai; Sidoti, A.; Camillocci, E. Solfaroli; Vari, R.; Veneziano, S.; Zanello, L.] INFN Sez Roma I, Rome, Italy. [Artoni, G.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Zorzi, G.; Dionisi, C.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Rossi, E.; Camillocci, E. Solfaroli; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Di Simone, A.; Liberti, B.; Marchese, F.; Mazzaferro, L.; Salamon, A.; Santonico, R.] INFN Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Cattani, G.; Di Ciaccio, A.; Di Simone, A.; Marchese, F.; Mazzaferro, L.; Messina, A.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Branchini, P.; Ceradini, F.; Di Luise, S.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Stanescu, C.] INFN Sez Roma Tre, Rome, Italy. [Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Luise, S.; Orestano, D.; Pastore, F.; Petrucci, F.] Univ Roma Tre, Dipartimento Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.; Lablak, S.] Univ Hassan 2, Fac Sci Ain Chock, Reseau Univ Phys Hautes Energies, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA Marrakech, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Abreu, H.; Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Bolnet, N. M.; Boonekamp, M.; Chevalier, L.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Gauthier, L.; Giraud, P. F.; Guyot, C.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Legendre, M.; Maiani, C.; Mal, P.; Ramos, J. A. Manjarres; Mansoulie, B.; Meyer, J-P.; Mijovic, L.; Morange, N.; Mountricha, E.; Hong, V. Nguyen Thi; Nicolaidou, R.; Ouraou, A.; Resende, B.; Royon, C. R.; Schoeffel, L.; Schune, Ph.; Schwindling, J.; Simard, O.; Virchaux, M.; Vranjes, N.; Xiao, M.; Xu, C.] CEA Saclay, Commissariat Energie Atom, DSM IRFU Inst Rech Lois Fondamentales Univers, F-91191 Gif Sur Yvette, France. [Chouridou, S.; Damiani, D. S.; Grillo, A. A.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Mitrevski, J.; Nielsen, J.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Beckingham, M.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Keller, J. S.; Lubatti, H. J.; Rompotis, N.; Rothberg, J.; Verducci, M.; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Duxfield, R.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Mayne, A.; Mcfayden, J. A.; Miyagawa, P. S.; Owen, S.; Paganis, E.; Suruliz, K.; Tovey, D. R.; Tsionou, D.; Tua, A.; Xu, D.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Holder, M.; Ibragimov, I.; Rammes, M.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Dawe, E.; Godfrey, J.; Kvita, J.; O'Neil, D. C.; Petteni, M.; Stelzer, B.; Tanasijczuk, A. J.; Trottier-McDonald, M.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Mayes, J. Backus; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Butler, B.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Grenier, P.; Hansson, P.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nelson, T. K.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Smith, D.; Strauss, E.; Su, D.; Wilson, M. G.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Batkova, L.; Blazek, T.; Federic, P.; Pecsy, M.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Ferencei, J.; Kladiva, E.; Seman, M.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Assamagan, K.; Aurousseau, M.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Carrillo-Montoya, G. D.; Hamilton, A.; Leney, K. J. C.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Asman, B.; Bendtz, K.; Bohm, C.; Clement, C.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Holmgren, S. O.; Johansen, M.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Papadelis, A.; Sellden, B.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Stockholm Univ, Dept Phys, Stockholm, Sweden. [Asman, B.; Bendtz, K.; Clement, C.; Gellerstedt, K.; Hellman, S.; Johansen, M.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Ahmad, A.; Arfaoui, S.; Devetak, E.; DeWilde, B.; Engelmann, R.; Farley, J.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Li, H.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Ahmad, A.; Arfaoui, S.; Devetak, E.; DeWilde, B.; Engelmann, R.; Farley, J.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Li, H.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Bartsch, V.; De Santo, A.; Martin-Haugh, S.; Potter, C. J.; Rose, A.; Salvatore, F.; Castillo, I. Santoyo; Sutton, M. R.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Bangert, A.; Black, C. W.; Cuthbert, C.; Patel, N.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Waugh, A. T.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Chu, M. L.; Hou, S.; Jamin, D. O.; Lee, S. C.; Lin, S. C.; Liu, D.; Mazini, R.; Meng, Z.; Ren, Z. L.; Soh, D. A.; Teng, P. K.; Wang, J.; Wang, S. M.; Weng, Z.; Zhang, D.; Zhou, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Harpaz, S. Behar; Kajomovitz, E.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; Vallecorsa, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Bella, G.; Benary, O.; Benhammou, Y.; Etzion, E.; Gershon, A.; Ginzburg, J.; Guttman, N.; Hod, N.; Munwes, Y.; Oren, Y.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Iliadis, D.; Kordas, K.; Kouskoura, V.; Nomidis, I.; Petridis, A.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, K.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yamazaki, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, K.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yamazaki, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Ishitsuka, M.; Jinnouchi, O.; Kanno, T.; Kuze, M.; Nagai, R.; Nobe, T.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Bailey, D. C.; Bain, T.; Brelier, B.; Cheung, S. L.; Dhaliwal, S.; Farooque, T.; Fatholahzadeh, B.; Gibson, A.; Guo, B.; Ilic, N.; Keung, J.; Krieger, P.; Orr, R. S.; Rezvani, R.; Rosenbaum, G. A.; Savard, P.; Sinervo, P.; Spreitzer, T.; Tardif, D.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Fortin, D.; Gingrich, D. M.; Koutsman, A.; Losty, M. J.; Nugent, I. M.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hanawa, K.; Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Kurata, M.; Nagai, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Napier, A.; Rolli, S.; Sliwa, K.; Todorova-Nova, S.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Loureiro, K. F.; Mendoza Navas, L.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Farrell, S.; Eschrich, I. Gough; Lankford, A. J.; Magnoni, L.; Mete, A. S.; Nelson, A.; Scannicchio, D. A.; Schernau, M.; Taffard, A.; Toggerson, B.; Unel, G.; Werth, M.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Pinamonti, M.; Shaw, K.; Soualah, R.] INFN Grp Collegato Udine, Udine, Italy. [Acharya, B. S.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Shaw, K.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Coggeshall, J.; Cortes-Gonzalez, A.; Errede, D.; Errede, S.; Lie, K.; Liss, T. M.; McCarn, A.; Neubauer, M. S.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Brenner, R.; Buszello, C. P.; Coniavitis, E.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Pelikan, D.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] CSIC, Valencia, Spain. [Axen, D.; Gay, C.; Gecse, Z.; Loh, C. W.; Mills, W. J.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Astbury, A.; Bansal, V.; Berghaus, F.; Courneyea, L.; Fincke-Keeler, M.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Lessard, J-R.; Marino, C. P.; Martyniuk, A. C.; McPherson, R. A.; Ouellette, E. A.; Plamondon, M.; Sobie, R.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Farrington, S. M.; Jones, G.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Kimura, N.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Alon, R.; Barak, L.; Bressler, S.; Citron, Z. H.; Duchovni, E.; Frank, T.; Gabizon, O.; Gross, E.; Groth-Jensen, J.; Klier, A.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Milstein, D.; Perez, G.; Roth, I.; Silbert, O.; Smakhtin, V.; Vitells, O.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Hernandez, A. M. Castaneda; Castaneda-Miranda, E.; Chen, X.; Di Mattia, A.; Dos Anjos, A.; Castillo, L. R. Flores; Gutzwiller, O.; Jared, R. C.; Ji, H.; Ju, X.; Kashif, L.; Ma, L. L.; Garcia, B. R. Mellado; Ming, Y.; Pan, Y. B.; Morales, M. I. Pedraza; Quayle, W. B.; Sarangi, T.; Wang, H.; Wiedenmann, W.; Wu, S. L.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Fleischmann, P.; Meyer, J.; Redelbach, A.; Siragusa, G.; Stroehmer, R.; Trefzger, T.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Barisonzi, M.; Becker, K.; Becks, K. H.; Boek, J.; Boek, T. T.; Braun, H. M.; Cornelissen, T.; Duda, D.; Fleischmann, S.; Flick, T.; Gerlach, P.; Glitza, K. W.; Gorfine, G.; Hamacher, K.; Harenberg, T.; Hirschbuehl, D.; Kalinin, S.; Kersten, S.; Khoroshilov, A.; Kohlmann, S.; Lantzsch, K.; Lenzen, G.; Maettig, P.; Mechtel, M.; Neumann, M.; Pataraia, S.; Sandhoff, M.; Sartisohn, G.; Schutes, J.; Sturm, P.; Wagner, W.; Wahlen, H.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany. [Adelman, J.; Baker, O. K.; Bedikian, S.; Almenar, C. Cuenca; Cummings, J.; Czyczula, Z.; Demers, S.; Garberson, F.; Golling, T.; Guest, D.; Henrichs, A.; Lagouri, T.; Lee, L.; Leister, A. G.; Loginov, A.; Sherman, D.; Tipton, P.; Wall, R.; Walsh, B.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Biscarat, C.; Cogneras, E.; Rahal, G.] Ctr Calcul Inst Natl Phys Nucl & Phys Particules, Villeurbanne, France. [Amorim, A.; Gomes, A.; Maio, A.; Pina, J.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amorim, A.; Gomes, A.; Maio, A.; Pina, J.] Univ Lisbon, CFNUL, P-1699 Lisbon, Portugal. [Bawa, H. S.; Gao, Y. S.; Lowe, A. J.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beloborodova, O.; Maximov, D. A.; Talyshev, A.; Tikhonov, Y. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Carvalho, J.; Fiolhais, M. C. N.; Oliveira, M.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Hernandez, A. M. Castaneda] UASLP, Dept Phys, San Luis Potosi, Mexico. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Demirkoz, B.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Dhullipudi, R.; Greenwood, Z. D.; Sawyer, L.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Wemans, A. Do Valle] Univ Nova Lisboa, Dep Fis, Caparica, Portugal. [Wemans, A. Do Valle] Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Dobson, E.] UCL, Dept Phys & Astron, London, England. [Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Kono, T.; Wildt, M. A.] Univ Hamburg, Inst Expt Phys, Hamburg, Germany. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Liang, Z.; Soh, D. A.; Weng, Z.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou, Peoples R China. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Park, W.; Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Pasztor, G.; Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Perez, K.] CALTECH, Pasadena, CA 91125 USA. [Richter-Was, E.] Jagiellonian Univ, Inst Phys, Krakow, Poland. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. RP Aad, G (reprint author), Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. RI Capua, Marcella/A-8549-2015; Tartarelli, Giuseppe Francesco/A-5629-2016; Fassi, Farida/F-3571-2016; la rotonda, laura/B-4028-2016; Zaitsev, Alexandre/B-8989-2017; Monzani, Simone/D-6328-2017; Grancagnolo, Francesco/K-2857-2015; Korol, Aleksandr/A-6244-2014; Karyukhin, Andrey/J-3904-2014; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Olshevskiy, Alexander/I-1580-2016; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Mora Herrera, Maria Clemencia/L-3893-2016; Maneira, Jose/D-8486-2011; KHODINOV, ALEKSANDR/D-6269-2015; Goncalo, Ricardo/M-3153-2016; Gauzzi, Paolo/D-2615-2009; Solodkov, Alexander/B-8623-2017; Tikhomirov, Vladimir/M-6194-2015; Chekulaev, Sergey/O-1145-2015; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; Carvalho, Joao/M-4060-2013; Mashinistov, Ruslan/M-8356-2015; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Wemans, Andre/A-6738-2012; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Tomasek, Lukas/G-6370-2014; Svatos, Michal/G-8437-2014; Chudoba, Jiri/G-7737-2014; Peleganchuk, Sergey/J-6722-2014; Santamarina Rios, Cibran/K-4686-2014; Bosman, Martine/J-9917-2014; Demirkoz, Bilge/C-8179-2014; Gutierrez, Phillip/C-1161-2011; Ventura, Andrea/A-9544-2015; Livan, Michele/D-7531-2012; Mitsou, Vasiliki/D-1967-2009; Joergensen, Morten/E-6847-2015; Mir, Lluisa-Maria/G-7212-2015; Riu, Imma/L-7385-2014; Cabrera Urban, Susana/H-1376-2015; Garcia, Jose /H-6339-2015; Della Pietra, Massimo/J-5008-2012; Cavalli-Sforza, Matteo/H-7102-2015; Negrini, Matteo/C-8906-2014; Ferrer, Antonio/H-2942-2015; Hansen, John/B-9058-2015; Grancagnolo, Sergio/J-3957-2015; spagnolo, stefania/A-6359-2012; Shmeleva, Alevtina/M-6199-2015; Camarri, Paolo/M-7979-2015; Gavrilenko, Igor/M-8260-2015; Robson, Aidan/G-1087-2011; Smirnova, Oxana/A-4401-2013; Fabbri, Laura/H-3442-2012; Villa, Mauro/C-9883-2009; Nemecek, Stanislav/G-5931-2014; Kepka, Oldrich/G-6375-2014; Jakoubek, Tomas/G-8644-2014; 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Moorhead, Gareth/B-6634-2009; Ma, Hong/F-2725-2011; Gordon, Howard/D-6734-2013; Rud, Vyacheslav/D-6838-2012; Alexa, Calin/F-6345-2010; Orlov, Ilya/E-6611-2012; Petrucci, Fabrizio/G-8348-2012; Annovi, Alberto/G-6028-2012; Brooks, William/C-8636-2013 OI Coccaro, Andrea/0000-0003-2368-4559; Abdelalim, Ahmed Ali/0000-0002-2056-7894; Capua, Marcella/0000-0002-2443-6525; Di Micco, Biagio/0000-0002-4067-1592; Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; Doria, Alessandra/0000-0002-5381-2649; Veloso, Filipe/0000-0002-5956-4244; Gomes, Agostinho/0000-0002-5940-9893; Fassi, Farida/0000-0002-6423-7213; la rotonda, laura/0000-0002-6780-5829; Osculati, Bianca Maria/0000-0002-7246-060X; Amorim, Antonio/0000-0003-0638-2321; Santos, Helena/0000-0003-1710-9291; Zaitsev, Alexandre/0000-0002-4961-8368; Monzani, Simone/0000-0002-0479-2207; Grancagnolo, Francesco/0000-0002-9367-3380; Korol, Aleksandr/0000-0001-8448-218X; Maio, Amelia/0000-0001-9099-0009; Fiolhais, Miguel/0000-0001-9035-0335; Karyukhin, Andrey/0000-0001-9087-4315; Anjos, Nuno/0000-0002-0018-0633; Smestad, Lillian/0000-0002-0244-8736; Giordani, Mario/0000-0002-0792-6039; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Olshevskiy, Alexander/0000-0002-8902-1793; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Maneira, Jose/0000-0002-3222-2738; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Goncalo, Ricardo/0000-0002-3826-3442; Gauzzi, Paolo/0000-0003-4841-5822; Solodkov, Alexander/0000-0002-2737-8674; Tikhomirov, Vladimir/0000-0002-9634-0581; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; Carvalho, Joao/0000-0002-3015-7821; Mashinistov, Ruslan/0000-0001-7925-4676; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Wemans, Andre/0000-0002-9669-9500; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Tomasek, Lukas/0000-0002-5224-1936; 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De, Kaushik/0000-0002-5647-4489; O'Shea, Val/0000-0001-7183-1205; Lee, Jason/0000-0002-2153-1519; Vanyashin, Aleksandr/0000-0002-0367-5666; Ferrando, James/0000-0002-1007-7816; La Rosa, Alessandro/0000-0001-6291-2142; Moraes, Arthur/0000-0002-5157-5686; Smirnov, Sergei/0000-0002-6778-073X; Conde Muino, Patricia/0000-0002-9187-7478; Andreazza, Attilio/0000-0001-5161-5759; Boyko, Igor/0000-0002-3355-4662; Kuleshov, Sergey/0000-0002-3065-326X; Stoicea, Gabriel/0000-0002-7511-4614; Doyle, Anthony/0000-0001-6322-6195; Pina, Joao /0000-0001-8959-5044; Moorhead, Gareth/0000-0002-9299-9549; Orlov, Ilya/0000-0003-4073-0326; Petrucci, Fabrizio/0000-0002-5278-2206; Annovi, Alberto/0000-0002-4649-4398; Brooks, William/0000-0001-6161-3570 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union; ERC, European Union; NSRF, European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; ISF, Israel; MINERVA, Israel; GIF, Israel; DIP, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; GRICES, Portugal; FCT, Portugal; MERYS (MECTS), Romania; MES of Russia, Russian Federation; ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MVZT, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America; Canton of Geneva, Switzerland FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; ISF, MINERVA, GIF, DIP and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW, Poland; GRICES and FCT, Portugal; MERYS (MECTS), Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MVZT, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. NR 66 TC 19 Z9 19 U1 7 U2 136 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JAN PY 2013 IS 1 AR 116 DI 10.1007/JHEP01(2013)116 PG 50 WC Physics, Particles & Fields SC Physics GA 098XY UT WOS:000315583600035 ER PT J AU Aad, G Abajyan, T Abbott, B Abdallah, J Khalek, SA Abdelalim, AA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Acharya, BS Adamczyk, L Adams, DL Addy, TN Adelman, J Adomeit, S Adragna, P Adye, T Aefsky, S Aguilar-Saavedra, JA Agustoni, M Aharrouche, M Ahlen, SP Ahles, F Ahmad, A Ahsan, M Aielli, G Akdogan, T Akesson, TPA Akimoto, G Akimov, AV Alam, MS Alam, MA Albert, J Albrand, S Aleksa, M Aleksandrov, IN Alessandria, F Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Aliev, M Alimonti, G Alison, J Allbrooke, BMM Allport, PP Allwood-Spiers, SE Almond, J Aloisio, A Alon, R Alonso, A Alonso, F Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Amelung, C Ammosov, VV Dos Santos, SPA Amorim, A Amram, N Anastopoulos, C Ancu, LS Andari, N Andeen, I Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Andrieux, ML Anduaga, XS Angelidakis, S Anger, P Angerami, A Anghinolfi, F Anisenkov, A Anjos, N Annovi, A Antonaki, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Aoun, S Bella, LA Apolle, R Arabidze, G Aracena, I Arai, Y Arce, ATH Arfaoui, S Arguin, JF Arik, E Arik, M Armbruster, AJ Arnaez, O Arnal, V Arnault, C Artamonov, A Artoni, G Arutinov, D Asai, S Ask, S Asman, B Asquith, L Assamagan, K Astbury, A Atkinson, M Aubert, B Auge, E Augsten, K Aurousseau, M Avolio, G Avramidou, R Axen, D Azuelos, G Azuma, Y Baak, MA Baccaglioni, G Bacci, C Bach, AM Bachacou, H Bachas, K Backes, M Backhaus, M Mayes, JB Badescu, E Bagnaia, P Bahinipati, S Bai, Y Bailey, DC Bain, T Baines, JT Baker, OK Baker, MD Baker, S Balek, P Banas, E Banerjee, P Banerjee, S Banfi, D Bangert, A Bansal, V Bansil, HS Barak, L Baranov, SP Galtieri, AB Barber, T Barberio, EL Barberis, D Barbero, M Bardin, DY Barillari, T Barisonzi, M Barklow, T Barlow, N Barnett, BM Barnett, RM Baroncelli, A Barone, G Barr, AJ Barreiro, F 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CA ATLAS Collaboration TI Search for direct chargino production in anomaly-mediated supersymmetry breaking models based on a disappearing-track signature in pp collisions at root s=7 TeV with the ATLAS detector SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering ID MASS-DEGENERATE; COLLIDERS; ENERGIES AB A search for direct chargino production in anomaly-mediated supersymmetry breaking scenarios is performed in p p collisions at root s = 7 TeV using 4.7 fb(-1) of data collected with the ATLAS experiment at the LHC. In these models, the lightest chargino is predicted to have a lifetime long enough to be detected in the tracking detectors of collider experiments. This analysis explores such models by searching for chargino decays that result in tracks with few associated hits in the outer region of the tracking system. 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P.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Gillberg, D.; Koffas, T.; Lacey, J.; Liu, C.; Marchand, J. F.; McCarthy, T. G.; Oakham, F. G.; Randrianarivony, K.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Anastopoulos, C.; Anghinolfi, F.; Avolio, G.; Baak, M. A.; Bachas, K.; Banfi, D.; Battistin, M.; Bellomo, M.; Beltramello, O.; Berge, D.; Bianchi, R. M.; Blanchot, G.; Bogaerts, J. A.; Boyd, J.; Bremer, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Catmore, J. R.; Cattai, A.; Cerri, A.; Barajas, C. A. Chavez; Childers, J. T.; Chromek-Burckhart, D.; Courneyea, L.; Danielsson, H. 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M.; Nakahama, Y.; Negri, G.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Ohm, C. C.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Petersen, J.; Piacquadio, G.; Pommes, K.; Poppleton, A.; Bueso, X. Portell; Poulard, G.; Prasad, S.; Raymond, M.; Rembser, C.; Dos Santos, D. Roda; Roe, S.; Salek, D.; Salzburger, A.; Savu, D. O.; Schlenker, S.; Schott, M.; Sfyrla, A.; Spigo, G.; Spiwoks, R.; Stewart, G. A.; Teischinger, F. A.; Ten Kate, H.; Torchiani, I.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van der Ster, D.; van Eldik, N.; Vandelli, W.; Veness, R.; Vinek, E.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Winklmeier, F.; Wotschack, J.; Byszewski, M.; Zajacova, Z.; Zwalinski, L.] CERN, Geneva, Switzerland. [Anderson, K. J.; Boveia, A.; Canelli, F.; Cheng, Y.; Choudalakis, G.; Fiascaris, M.; Gardner, R. W.; Plante, I. Jen-La; Kapliy, A.; Li, H. L.; Melachrinos, C.; Merritt, F. S.; Meyer, C.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Shochet, M. J.; Tompkins, L.; Tuggle, J. M.; Vukotic, I.; Webster, J. S.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Diaz, M. A.; Olivares Pino, S. A.; Quinonez, F.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Carquin, E.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Jin, S.; Lu, F.; Ouyang, Q.; Ruan, X.; Shan, L. Y.; Yao, L.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Han, L.; Jiang, Y.; Li, S.; Liu, M.; Liu, Y.; Peng, H.; Wang, H.; Wu, Y.; Xu, C.; Zhang, D.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Feng, C.; Ge, P.; Meng, Z.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Toro, R. Camacho; Cinca, D.; Donini, J.; Febbraro, R.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Vazeille, F.] Univ Clermont Ferrand 2, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Toro, R. Camacho; Cinca, D.; Donini, J.; Febbraro, R.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Vazeille, F.] Univ Blaise Pascal, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Toro, R. Camacho; Cinca, D.; Donini, J.; Febbraro, R.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Vazeille, F.] Univ Clermont Ferrand 2, Photochim Mol & Macromol Lab, CNRS, IN2P3, F-63177 Clermont Ferrand, France. [Altheimer, A.; Andeen, I.; Angerami, A.; Brooijmans, G.; Chen, Y.; Dodd, J.; Grau, N.; Guo, J.; Hu, D.; Hughes, E. W.; Nikiforou, N.; Parsons, J. A.; Penson, A.; Perez, K.; Reale, V. Perez; Scherzer, M. I.; Spousta, M.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Williams, E.; Willis, W.; Wulf, E.; Zivkovic, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Boelaert, N.; Dam, M.; Gregersen, K.; Hansen, J. R.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Heisterkamp, S.; Jakobsen, S.; Loevschall-Jensen, A. E.; Jez, P.; Joergensen, M. D.; Kadlecik, P.; Klinkby, E. B.; Lundquist, J.; Mackeprang, R.; Mehlhase, S.; Petersen, T. C.; Simonyan, M.; Thomsen, L. A.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; Fazio, S.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Morello, G.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] INFN Grp Collegato Conseza, Conseza, Italy. [Capua, M.; Crosetti, G.; Fazio, S.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Morello, G.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Banas, E.; Blocki, J.; de Renstrom, P. A. Bruckman; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Malecki, P.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Turala, M.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.; Zemla, A.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Yagci, K. Dindar; Firan, A.; Hoffman, J.; Joffe, D.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Rios, R. R.; Sekula, S. J.; Stroynowski, R.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Ahsan, M.; Izen, J. M.; Lou, X.; Reeves, K.; Wong, W. C.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Kuutmann, F. Bergeaas; Bloch, I.; Dassoulas, J. A.; Dietrich, J.; Ehrenfeld, W.; Ferrara, V.; Fischer, G.; Friedrich, C.; Glazov, A.; Goebel, M.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Gosdzik, B.; Grahn, K-J.; Gregor, I. M.; Hiller, K. H.; Huettmann, A.; Belenguer, M. Jimenez; Johnert, S.; Karnevskiy, M.; Katzy, J.; Kono, T.; Kuhl, T.; Lange, C.; Lobodzinska, E.; Ludwig, D.; Medinnis, M.; Moenig, K.; Naumann, T.; Cavalcanti, T. Perez; Petschull, D.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Ziu, H.] DESY, Hamburg, Germany. [Kuutmann, F. Bergeaas; Bloch, I.; Dassoulas, J. A.; Dietrich, J.; Ehrenfeld, W.; Ferrara, V.; Fischer, G.; Friedrich, C.; Glazov, A.; Goebel, M.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Gosdzik, B.; Grahn, K-J.; Gregor, I. M.; Hiller, K. H.; Huettmann, A.; Belenguer, M. Jimenez; Johnert, S.; Karnevskiy, M.; Katzy, J.; Kono, T.; Kuhl, T.; Lange, C.; Lobodzinska, E.; Ludwig, D.; Medinnis, M.; Moenig, K.; Naumann, T.; Cavalcanti, T. Perez; Petschull, D.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Ziu, H.] DESY, Zeuthen, Germany. [Bunse, M.; Esch, H.; Goessling, C.; Hirsch, F.; Jung, C. A.; Klingenberg, R.; Reisinger, I.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Czodrowski, P.; Friedrich, F.; Goepfert, T.; Kobel, M.; Leonhardt, K.; Ludwig, A.; Mader, W. F.; Morgenstern, M.; Prudent, X.; Rudolph, C.; Schnoor, U.; Schwierz, R.; Seifert, F.; Steinbach, P.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Ebenstein, W. L.; Fowler, A. J.; Ko, B. R.; Kotwal, A.; Kruse, M. K.; Oh, S. H.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Buckley, A. G.; Clark, P. J.; Debenedetti, C.; Harrington, R. D.; Martin, V. J.; O'Brien, B. J.; Schaelicke, A.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Cerutti, F.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.; Volpi, G.] INFN Lab Nazl Frascati, Frascati, Italy. [Aad, G.; Ahles, F.; Barber, T.; Bernhard, R.; Boehler, M.; Bruneliere, R.; Christov, A.; Consorti, V.; Fehling-Kaschek, M.; Flechl, M.; Hartert, J.; Herten, G.; Horner, S.; Jakobs, K.; Janus, M.; Kononov, A. I.; Kuehn, S.; Lai, S.; Landgraf, U.; Lohwasser, K.; Ludwig, I.; Ludwig, J.; Mahboubi, K.; Mohr, W.; Nilsen, H.; Parzefall, U.; Rammensee, M.; Rave, T. C.; Rurikova, Z.; Schmidt, E.; Schumacher, M.; Siegert, F.; Stoerig, K.; Sundermann, J. E.; Temming, K. K.; Thoma, S.; Tsiskaridze, V.; Venturi, M.; Vivarelli, I.; von Radziewski, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Winkelmann, S.; Xie, S.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Abdelalim, A. A.; Alexandre, G.; Backes, M.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; Blondel, A.; Bucci, F.; Clark, A.; Dao, V.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Iacobucci, G.; La Rosa, A.; Lister, A.; Latour, B. Martin dit; Mermod, P.; Herrera, C. Mora; Nektarijevic, S.; Nessi, M.; Nikolics, K.; Pasztor, G.; Picazio, A.; Pohl, M.; Rosbach, K.; Rosselet, L.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Beccherle, R.; Caso, C.; Dameri, M.; Darbo, G.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] INFN Sez Genova, Genoa, Italy. [Barberis, D.; Caso, C.; Dameri, M.; Parodi, A. Ferretto; Gagliardi, G.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Chikovani, L.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Khubua, J.; Mchedlidze, G.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Bussey, P.; Buttar, C. M.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Edwards, N. C.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Kar, D.; Kenyon, M.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Robson, A.; Saxon, D. H.; Smith, K. M.; Denis, R. D. St.; Steele, C.; Thompson, A. S.; Wraight, K.; Wright, M.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bierwagen, K.; Blumenschein, U.; Brandt, O.; Erdmann, J.; Evangelakou, D.; George, M.; Grosse-Knetter, J.; Guindon, S.; Hamer, M.; Hensel, C.; Keil, M.; Knue, A.; Kohn, F.; Krieger, N.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Mann, A.; Meyer, J.; Morel, J.; Nackenhorst, O.; Pashapour, S.; Quadt, A.; Roe, A.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Uhrmacher, M.; Schroeder, T. Vazquez; Weber, P.; Weingarten, J.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Andrieux, M-L.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Stark, J.; Sun, X.; Wang, J.; Weydert, C.] Univ Grenoble 1, Lab Phys Subatom & Cosmol, Grenoble, France. [Albrand, S.; Andrieux, M-L.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Stark, J.; Sun, X.; Wang, J.; Weydert, C.] CNRS, IN2P3, Grenoble, France. [Albrand, S.; Andrieux, M-L.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Stark, J.; Sun, X.; Wang, J.; Weydert, C.] Inst Natl Polytech Grenoble, F-38031 Grenoble, France. [Addy, T. N.; Harvey, A.; McFarlane, K. W.; Shin, T.; Vassilakopoulos, V. I.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Belloni, A.; Catastini, P.; Conti, G.; Franklin, M.; Huth, J.; Jeanty, L.; Kagan, M.; Mateos, D. Lopez; Outschoorn, V. Martinez; Mercurio, K. M.; Mills, C.; Morii, M.; Skottowe, H. P.; Smith, B. C.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Anders, G.; Andrei, V.; Davygora, Y.; Dietzsch, T. A.; Dunford, M.; Geweniger, C.; Hanke, P.; Henke, M.; Khomich, A.; Kluge, E. -E.; Lang, V. S.; Lendermann, V.; Lepold, F.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H-C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Kugel, A.; Maenner, R.; Schroer, N.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Cwetanski, P.; Evans, H.; Gagnon, P.; Jain, V.; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Price, D.; Whittington, D.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Epp, B.; Jussel, P.; Kneringer, E.; Kuhn, D.; Lukas, W.; Rudolph, G.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Behera, P. K.; Limper, M.; Mallik, U.; Pylypchenko, Y.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Rosenberg, E. I.; Ruiz-Martinez, A.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Aleksandrov, I. N.; Bardin, D. Y.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Chepakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Grigalashvili, N.; Huseynov, N.; Kalinovskaya, L. V.; Kazarinov, M. Y.; Kekelidze, G. D.; Kharchenko, D.; Khramov, E.; Kolesnikov, V.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Pozdnyakov, V.; Rumyantsev, L.; Rusakovich, N. A.; Sadykov, R.; Shiyakova, M.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.; Zimin, N. I.] Joint Inst Nucl Res Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Arai, Y.; Doi, Y.; Haruyama, T.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Makida, Y.; Manabe, A.; Mitsui, S.; Nagano, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Trocme, B.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Hayakawa, T.; King, M.; Kishimoto, T.; Kitamura, T.; Kurashige, H.; Matsushita, T.; Ochi, A.; Suzuki, Y.; Takeda, H.; Tani, K.; Watanabe, I.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Sasao, N.; Sumida, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Khodinov, A.; Oda, S.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Davidson, R.; de Mora, L.; Dearnaley, W. J.; Fox, H.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Bianco, M.; Cataldi, G.; Chiodini, G.; Gorini, E.; Grancagnolo, F.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] INFN Sez Lecce, Lecce, Italy. [Bianco, M.; Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Greenshaw, T.; Gwilliam, C. B.; Hayward, H. S.; Jackson, J. N.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kluge, T.; Kretzschmar, J.; Laycock, P.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Sellers, G.; Vossebeld, J. H.; Waller, P.; Wrona, B.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Dolenc, I.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Dolenc, I.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia. [Adragna, P.; Bona, M.; Carter, A. A.; Cerrito, L.; Eisenhandler, E.; Ellis, K.; Goddard, J. R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Poll, J.; Rizvi, E.; Salamanna, G.; Castanheira, M. Teixeira Dias; Wiglesworth, C.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Alam, M. A.; Berry, T.; Boisvert, V.; Brooks, T.; Cantrill, R.; Cowan, G.; Duguid, L.; Edwards, C. A.; George, S.; Goncalo, R.; Hayden, D.; Vazquez, J. G. Panduro; Pastore, Fr.; Rose, M.; Spano, F.; Strong, J. A.; Teixeira-Dias, P.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Baker, S.; Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Chislett, R. T.; Christidi, I. A.; Cooper, B. D.; Davison, A. R.; Dobson, E.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Lambourne, L.; Monk, J.; Nash, M.; Nurse, E.; Prabhu, R.; Sherwood, P.; Simmons, B.; Taylor, C.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Cavalleri, P.; Chareyre, E.; Davignon, O.; De Cecco, S.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Lafarge, B.; Laplace, S.; Le Dortz, O.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph.; Theveneaus-Pelzer, T.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Cavalleri, P.; Chareyre, E.; Davignon, O.; De Cecco, S.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Lafarge, B.; Laplace, S.; Le Dortz, O.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph.; Theveneaus-Pelzer, T.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Cavalleri, P.; Chareyre, E.; Davignon, O.; De Cecco, S.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Lafarge, B.; Laplace, S.; Le Dortz, O.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph.; Theveneaus-Pelzer, T.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Alonso, A.; Bocchetta, S. S.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Jarlskog, G.; Lundberg, B.; Lytken, E.; Meirose, B.; Mjornmark, J. U.; Smirnova, O.] Lund Univ, Fysiska Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Gasman, C.; Labarga, L.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Aharrouche, M.; Arnaez, O.; Blum, W.; Buescher, V.; Caputo, R.; Eckweiler, S.; Edmonds, K.; Ellinghaus, F.; Ertel, E.; Fiedler, F.; Fleckner, J.; Goeringer, C.; Handel, C.; Hohlfeld, M.; Hsu, P. J.; Ji, W.; Kawamura, G.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lungwitz, M.; Maettig, S.; Masetti, L.; Meyer, C.; Moreno, D.; Mueller, T.; Neusiedl, A.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schroeder, C.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Almond, J.; Borri, M.; Brown, G.; Chavda, V.; Cox, B. E.; Da Via, C.; Duerdoth, I. P.; Forti, A.; Howarth, J.; Ibbotson, M.; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Marx, M.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Pilkington, A. D.; Robinson, J. E. M.; Schwanenberger, C.; Snow, S. W.; Watts, S.; Woudstra, M. J.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aoun, S.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Li, S.; Maurer, J.; Monnier, E.; Odier, J.; Pralavorio, P.; Rozanov, A.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aoun, S.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Li, S.; Maurer, J.; Monnier, E.; Odier, J.; Pralavorio, P.; Rozanov, A.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Brau, B.; Colon, U.; Dallapiccola, C.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Caron, B.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Dobbs, M.; Dufour, M-A.; Klemetti, M.; Mc Donald, J.; Robertson, S. H.; Rios, C. Santamarina; Schram, M.; Stockton, M. C.; Vachon, B.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Davidson, N.; Diglio, S.; Hamano, K.; Jennens, D.; Kubota, T.; Limosani, A.; Moorhead, G. F.; Hanninger, G. Nunes; Phan, A.; Shao, Q. T.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Volpi, M.; White, M. J.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Armbruster, A. J.; Borroni, S.; Chapman, J. W.; Cirilli, M.; Dai, T.; Diehl, E. B.; Ferretti, C.; Godfarb, S.; Harper, D.; Levin, D.; Li, X.; Liu, H.; Liu, J. B.; Liu, L.; Mc Kee, S. P.; Neal, H. A.; Panikashvili, N.; Purdham, J.; Qian, J.; Scheirich, D.; Thun, R. P.; Walch, S.; Wilson, A.; Wooden, C.; Wu, Y.; Yang, H.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Fedorko, W.; Hauser, R.; Heim, S.; Holzbauer, J. L.; Huston, J.; Koll, J.; Linnemann, J. T.; Mangeard, P. S.; Martin, B.; Miller, R. J.; Pope, B. G.; Schwienhorst, R.; Stelzer, H. J.; Tollefson, K.; True, P.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alessandria, F.; Alimonti, G.; Andreazza, A.; Baccaglioni, G.; Besana, M. I.; Broggi, F.; Carminati, L.; Cavalli, D.; Citterio, M.; Consonni, S. M.; Costa, G.; Fanti, M.; Favareto, A.; Giugni, D.; Koletsou, I.; Lari, T.; Mandelli, L.; Mazzanti, M.; Meloni, F.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Rivoltella, G.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Vegni, G.; Volpini, G.] INFN Sez Milano, Milan, Italy. [Andreazza, A.; Besana, M. I.; Carminati, L.; Consonni, S. M.; Fanti, M.; Favareto, A.; Meloni, F.; Perini, L.; Pizio, C.; Ragusa, F.; Rivoltella, G.; Simoniello, R.; Turra, R.; Vegni, G.] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Satsounkevitch, I.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus. [Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Banerjee, P.; Bouchami, J.; Davies, M.; Giunta, M.; Leroy, C.; Martin, J. P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinitov, H.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.] Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.] Moscow Engn & Phys Inst MEPhI, Moscow, Russia. [Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. 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G.; Nagel, M.; Nisius, R.; Oberlack, H.; Pahl, C.; Pospelov, G. E.; Potrap, I. N.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph; Stern, S.; Stonjek, S.; Vanadia, M.; von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.; Zhuravlov, V.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Shimizu, S.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Shimizu, S.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Capasso, L.; Carlino, G.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; della Volpe, L.; Di Donato, C.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Musto, E.; Patricelli, S.; Sanchez, A.; Sekhniaidze, G.] INFN Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Capasso, L.; Chiefari, G.; della Volpe, L.; Di Donato, C.; Giordano, R.; Merola, L.; Musto, E.; Patricelli, S.; Sanchez, A.] Univ Naples Federico II, Dipartimento Sci Fisiche, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Chelstowska, M. A.; de Groot, N.; Filthaut, F.; Klok, P. F.; Koenig, A. C.; Koetsveld, F.; Raas, M.; Salvucci, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Doxiadis, A. D.; Ferrari, P.; Garitaonandia, H.; Geerts, D. A. A.; Gosselink, M.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kayl, M. S.; Klous, S.; Kluit, P.; Koffeman, E.; Krasznahorkay, A.; Lee, H.; Lenz, T.; Linde, F.; Luijckx, G.; Mahlstedt, J.; Massaro, G.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Pani, P.; Rijpstra, M.; Ruckstuhl, N.; Ta, D.; Tsiakiris, M.; Turlay, E.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van der Poel, E.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.] Nikhef Natl Inst Subatom Phys, Amsterdam, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Doxiadis, A. D.; Ferrari, P.; Garitaonandia, H.; Geerts, D. A. A.; Gosselink, M.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kayl, M. S.; Klous, S.; Kluit, P.; Koffeman, E.; Krasznahorkay, A.; Lee, H.; Lenz, T.; Linde, F.; Luijckx, G.; Mahlstedt, J.; Massaro, G.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Pani, P.; Rijpstra, M.; Ruckstuhl, N.; Ta, D.; Tsiakiris, M.; Turlay, E.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van der Poel, E.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.] Univ Amsterdam, Amsterdam, Netherlands. [Calkins, R.; Chakraborty, D.; Cole, S.; de Lima, J. G. Rocha; Suhr, C.; Yurkewicz, A.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL USA. [Anisenkov, A.; Beloborodova, O.; Bobrovnikov, V. B.; Bogdanchikov, A.; Kazanin, V. A.; Kolachev, G. M.; Korol, A.; Malyshev, V.; Maslennikov, A. L.; Orlov, I.; Peleganchuk, S. V.; Schamov, A. G.; Skovpen, K.; Soukharev, A.; Talyshev, A.; Tikhonov, Y. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Budick, B.; Casadei, D.; Cranmer, K.; Haas, A.; van Huysduynen, L. Hooft; Kaplan, B.; Konoplich, R.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.; Prokofiev, K.; Zhao, L.] NYU, Dept Phys, New York, NY 10003 USA. [Fisher, M. J.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Rahimi, A. M.; Strang, M.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Gutierrez, P.; Jana, D. K.; Marzin, A.; Meera-Lebbai, R.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Snow, J.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Khanov, A.; Rizatdinova, F.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Hamal, P.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Potter, C. T.; Ptacek, E.; Radloff, P.; Reinsch, A.; Searcy, J.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Andari, N.; Arnault, C.; Auge, E.; Barrillon, P.; Benoit, M.; Binet, S.; Bourdarios, C.; De La Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Matricon, P.; Niedercorn, F.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Ruan, X.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Teinturier, M.; Veillet, J. J.; Wicek, F.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Andari, N.; Arnault, C.; Auge, E.; Barrillon, P.; Benoit, M.; Binet, S.; Bourdarios, C.; De La Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Matricon, P.; Niedercorn, F.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Ruan, X.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Teinturier, M.; Veillet, J. J.; Wicek, F.; Zerwas, D.; Zhang, Z.] CNRS, IN2P3, F-91405 Orsay, France. [Hanagaki, K.; Hirose, M.; Lee, J. S. H.; Meguro, T.; Nomachi, M.; Okaraura, W.; Sugaya, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Buran, T.; Cameron, D.; Gjelsten, B. K.; Gramstad, E.; Lund, E.; Ould-Saada, F.; Pajchel, K.; Read, A. L.; Rohne, O.; Samset, B. H.; Smestad, L.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Apolle, R.; Barr, A. J.; Boddy, C. R.; Brandt, G.; Buchanan, J.; Buckingham, R. M.; Cooper-Sarkar, A. M.; Dafinca, A.; Davies, E.; Gallas, E. J.; Gwenlan, C.; Hall, D.; Hays, C. P.; Howard, J.; Huffman, T. B.; Issever, C.; King, R. S. B.; Kogan, L. A.; Korn, A.; Larner, A.; Lewis, A.; Liang, Z.; Livermore, S. S. A.; Mattravers, C.; Nickerson, R. B.; Pinder, A.; Robichaud-Veronneau, A.; Ryder, N. C.; Short, D.; Tseng, J. C-L; Vickey, T.; Viehhauser, G. H. A.; Weidberg, A. R.; Whitehead, S. R.; Young, C. J.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Colombo, T.; Conta, C.; Ferrari, R.; Franchino, S.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Uslenghi, M.; Vercesi, V.] INFN Sez Pavia, Pavia, Italy. [Colombo, T.; Conta, C.; Franchino, S.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.; Uslenghi, M.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Alison, J.; Brendlinger, K.; Degenhardt, J.; Dressnandt, N.; Fratina, S.; Hines, E.; Hong, T. M.; Jackson, B.; Keener, P. T.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Newcomer, F. M.; Olivito, D.; Ospanov, R.; Reece, R.; Saxon, J.; Schaefer, D.; Stahlman, J.; Thomson, E.; Van Berg, R.; Wagner, P.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Bertolucci, F.; Cascella, M.; Cavasinni, V.; Crescioli, F.; Del Prete, T.; Dotti, A.; Roda, C.; Sarri, F.; White, S.; Zinonos, Z.] INFN Sez Pisa, Pisa, Italy. [Bertolucci, F.; Cascella, M.; Cavasinni, V.; Crescioli, F.; Del Prete, T.; Dotti, A.; Roda, C.; Sarri, F.; White, S.; Zinonos, Z.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Boudreau, J.; Cleland, W.; Escobar, C.; Kittelmann, T.; Mueller, J.; Prieur, D.; Savinov, V.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Anjos, N.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Do Valle Wemans, A.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Jorge, P. M.; Lopes, L.; Machado Miguens, J.; Maio, A.; Maneira, J.; Oliveira, M.; Onofre, A.; Palma, A.; Pina, J.; Pinto, B.; Sontos, H.; Saraiva, J. G.; Silva, J.; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. [Bohm, J.; Chudoba, J.; Gallus, P.; Gunther, J.; Jakoubek, T.; Juranek, V.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Marcisovsky, M.; Mikestikova, M.; Myska, M.; Nemecek, S.; Ruzicka, P.; Schovancova, J.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Tic, T.; Valenta, J.; Vrba, V.; Zeman, M.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Balek, P.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Kodys, P.; Leitner, R.; Novakova, J.; Rybar, M.; Spousta, M.; Strachota, P.; Suk, M.; Sykora, T.; Tas, P.; Valkar, S.; Vorobel, V.; Wilhelm, I.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Augsten, K.; Holy, T.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Kral, V.; Krejci, F.; Pospisil, S.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solar, M.; Solc, J.; Sopko, V.; Sopko, B.; Stekl, I.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.] Czech Tech Univ, Prague, Czech Republic. [Ammosov, V. V.; Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Ivashin, A. V.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.; Zmouchko, V. V.] Inst High Energy Phys, State Res Ctr, Protvino, Russia. [Adye, T.; Apolle, R.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Gillman, A. R.; Haywood, S. J.; Kirk, J.; Mattravers, C.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Nash, M.; Norton, P. R.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Benslama, K.; Smit, G. V. Ybeles] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Shiga, Japan. [Anulli, F.; Artoni, G.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Pedis, D.; De Salvo, A.; De Zorzi, G.; Dionisi, C.; Falciano, S.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; La Sterzo, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Rossi, E.; Tehrani, F. Safai; Sidoti, A.; Camillocci, E. Solfaroli; Vari, R.; Veneziano, S.; Zanello, L.] INFN Sez Roma I, Rome, Italy. [Artoni, G.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Zorzi, G.; Dionisi, C.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; La Sterzo, F.; Luci, C.; Messina, A.; Rossi, E.; Camillocci, E. Solfaroli; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Di Simone, A.; Liberti, B.; Marchese, F.; Mazzaferro, L.; Salamon, A.; Santonico, R.] INFN Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Cattani, G.; Di Ciaccio, A.; Di Simone, A.; Marchese, F.; Mazzaferro, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Branchini, P.; Ceradini, F.; Di Luise, S.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Stanescu, C.] INFN Sez Roma Tre, Rome, Italy. [Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Luise, S.; Orestano, D.; Pastore, F.; Petrucci, F.] Univ Roma Tre, Dipartimento Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.; Lablak, S.] Univ Hassan 2, Fac Sci Ain Chock, Reseau Univ Phys Hautes Energies, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, Lphea Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Abreu, H.; Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Bolnet, N. M.; Boonekamp, M.; Chevalier, L.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Gauthier, L.; Giraud, P. F.; Guyot, C.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Legendre, M.; Maiani, C.; Mal, P.; Ramos, J. A. Manjarres; Mansoulie, B.; Meyer, J. P.; Mijovic, L.; Morange, N.; Mountricha, E.; Hong, V. Nguyen Thu; Nicolaidou, R.; Ouraou, A.; Resende, B.; Royon, C. R.; Schoeffel, L.; Schune, Ph.; Schwindling, J.; Simard, O.; Virchaux, M.; Vranjes, N.; Xiao, M.; Xu, C.] CEA Saclay, Commissariat Energie Atom, DSM IRFU Inst Rech Lois Fondamentales Univers, F-91191 Gif Sur Yvette, France. [Chouridou, S.; Damiani, D. S.; Grillo, A. A.; Hare, G. A.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Mitrevski, J.; Nielsen, J.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Beckingham, M.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Keller, J. S.; Lubatti, H. J.; Rompotis, N.; Rothberg, J.; Verducci, M.; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Cote, D.; Donszelmann, T. Cuhadar; Dawson, I.; Duxfield, R.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Mayne, A.; Mcfayden, J. A.; Miyagawa, P. S.; Owen, S.; Paganis, E.; Suruliz, K.; Tovey, D. R.; Tsionou, D.; Tua, A.; Xu, D.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Holder, M.; Ibragimov, I.; Rammes, M.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Dawe, E.; Godfrey, J.; Kvita, J.; O'Neil, D. C.; Petteni, M.; Stelzer, B.; Tanasijczuk, A. J.; Trottier-McDonald, M.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Mayes, J. Backus; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Butler, B.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Grenier, P.; Hansson, P.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nelson, T. K.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Smith, D.; Strauss, E.; Su, D.; Wilson, M. G.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Batkova, L.; Blazek, T.; Federic, P.; Pecsy, M.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Ferencei, J.; Kladiva, E.; Seman, M.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Aurousseau, M.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Hamilton, A.; Leney, K. J. C.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Asman, B.; Bendtz, K.; Bohm, C.; Clement, C.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Holmgren, S. O.; Johansen, M.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Papadelis, A.; Sellden, B.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Stockholm Univ, Dept Phys, Stockholm, Sweden. [Asman, B.; Bendtz, K.; Clement, C.; Gellerstedt, K.; Hellman, S.; Johansen, M.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Ahmad, A.; Arfaoui, S.; Devetak, E.; DeWilde, B.; Engelmann, R.; Farley, J.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Li, H.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybyehev, D.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Ahmad, A.; Arfaoui, S.; Devetak, E.; DeWilde, B.; Engelmann, R.; Farley, J.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Li, H.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybyehev, D.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Bartsch, V.; De Santo, A.; Martin-Haugh, S.; Potter, C. J.; Rose, A.; Salvatore, F.; Sutton, M. R.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Bangert, A.; Cuthbert, C.; Patel, N.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Waugh, A. T.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Chu, M. L.; Hou, S.; Jamin, D. O.; Lee, S. C.; Lin, S. C.; Liu, D.; Mazini, R.; Meng, Z.; Ren, Z. L.; Soh, D. A.; Teng, P. K.; Wang, H.; Wang, J.; Wang, S. M.; Weng, Z.; Zhang, D.; Zhou, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Harpaz, S. Behar; Kajomovitz, E.; Kopeliansky, R.; Hozen, Y.; Tarem, S.; Vallecorsa, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Bella, G.; Benary, O.; Benhammou, Y.; Etzion, E.; Gershon, A.; Ginzburg, J.; Guttman, N.; Hod, N.; Munwes, Y.; Oren, Y.; Reinherz-Aronis, E.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Iliadis, D.; Kordas, K.; Kouskoura, V.; Nomidis, I.; Petridis, A.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, K.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yamazaki, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, K.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yamazaki, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Ishitsuka, M.; Jinnouchi, O.; Kanno, T.; Kuze, M.; Nagai, R.; Nobe, T.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Bailey, D. C.; Bain, T.; Brelier, B.; Cheung, S. L.; Dhaliwal, S.; Farooque, T.; Fatholahzadeh, B.; Gibson, A.; Guo, B.; Ilic, N.; Keung, J.; Krieger, P.; Martens, F. K.; Orr, R. S.; Rezvani, R.; Rosenbaum, G. A.; Savard, P.; Sinervo, P.; Spreitzer, T.; Tardif, D.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Canepa, A.; Chekulaev, S. V.; Fortin, D.; Gingrich, D. M.; Koutsman, A.; Losty, M. J.; Nugent, I. M.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hanawa, K.; Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Kurata, M.; Nagai, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Napier, A.; Rolli, S.; Sliwa, K.; Todorova-Nova, S.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Loureiro, K. F.; Mendoza Navas, L.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Deng, J.; Farrell, S.; Eschrich, I. Gough; Lankford, A. J.; Magnoni, L.; Mete, A. S.; Nelson, A.; Scannicchio, D. A.; Schernau, M.; Taffard, A.; Toggerson, B.; Unel, G.; Werth, M.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Pinamonti, M.; Shaw, K.; Soualah, R.] INFN Grp Collegato Udine, Udine, Italy. [Acharya, B. S.; Alhroob, M.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Coggeshall, J.; Cortes-Gonzalez, A.; Errede, D.; Errede, S.; Lie, K.; Liss, T. M.; McCarn, A.; Neubauer, M. S.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Brenner, R.; Buszello, C. P.; Coniavitis, E.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Pelikan, D.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] CSIC, Valencia, Spain. [Axen, D.; Gay, C.; Gecse, Z.; Loh, C. W.; Mills, W. J.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Astbury, A.; Bansal, V.; Berghaus, F.; Fincke-Keeler, M.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Lessard, J-R.; Marino, C. P.; Martyniuk, A. C.; McPherson, R. A.; Ouellette, E. A.; Plamondon, M.; Sobie, R.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Farrington, S. M.; Jones, G.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Kimura, N.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Alon, R.; Barak, L.; Bressler, S.; Citron, Z. H.; Duchovni, E.; Frank, T.; Gabizon, O.; Gross, E.; Groth-Jensen, J.; Klier, A.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Milstein, D.; Roth, I.; Silbert, O.; Smakhtin, V.; Vitells, O.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Carrillo-Montoya, G. D.; Hernandez, A. M. 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T.; Wagner, W.; Wahlen, H.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany. [Adelman, J.; Baker, O. K.; Bedikian, S.; Almenar, C. Cuenca; Czyczula, Z.; Demers, S.; Garberson, F.; Golling, T.; Guest, D.; Henrichs, A.; Lagouri, T.; Lee, L.; Loginov, A.; Sherman, D.; Tipton, P.; Wall, R.; Walsh, B.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Biscarat, C.; Cogneras, E.; Rahal, G.] Inst Natl Phys Nucl & Phys Particules IN2P3, Ctr Calcul, Villeurbanne, France. [Amorim, A.; Gomes, A.; Maio, A.; Pina, J.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amorim, A.; Gomes, A.; Maio, A.; Pina, J.] Univ Lisbon, CFNUL, P-1699 Lisbon, Portugal. [Bawa, H. S.; Gao, Y. S.; Lowe, A. J.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beloborodova, O.; Talyshev, A.; Tikhonov, Y. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Canelli, F.] Fermilab Natl Accelerator Lab, Batavia, IL USA. [Carvalho, J.; Fiolhais, M. C. N.; Oliveira, M.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Hernandez, A. M. Castaneda] UASLP, Dept Phys, San Luis Potosi, Mexico. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Demirkoz, B.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Dhullipudi, K.; Greenwood, Z. D.; Sawyer, L.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Do Valle Wemans, A.] Univ Nova Lisboa, Dep Fis, Fac Ciencias & Tecnol, Caparica, Portugal. [Do Valle Wemans, A.] Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, Caparica, Portugal. [Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Kono, T.; Wildt, M. A.] Univ Hamburg, Inst Expt Phys, Hamburg, Germany. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Liang, Z.; Soh, D. A.; Weng, Z.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou, Peoples R China. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Park, W.; Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Pasztor, G.; Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Perez, K.] CALTECH, Pasadena, CA 91125 USA. [Richter-Was, E.] Jagiellonian Univ, Inst Phys, Krakow, Poland. [Yacoob, S.] Univ KwaZalu Natal, Discipline Phys, Durban, South Africa. RP Aad, G (reprint author), Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. RI Livan, Michele/D-7531-2012; Amorim, Antonio/C-8460-2013; Vanyashin, Aleksandr/H-7796-2013; Ferrando, James/A-9192-2012; Casadei, Diego/I-1785-2013; La Rosa, Alessandro/I-1856-2013; Moraes, Arthur/F-6478-2010; Smirnov, Sergei/F-1014-2011; Conde Muino, Patricia/F-7696-2011; Andreazza, Attilio/E-5642-2011; Boyko, Igor/J-3659-2013; Kuleshov, Sergey/D-9940-2013; Stoicea, Gabriel/B-6717-2011; Fazio, Salvatore /G-5156-2010; Doyle, Anthony/C-5889-2009; Pina, Joao /C-4391-2012; Moorhead, Gareth/B-6634-2009; Ma, Hong/F-2725-2011; Gordon, Howard/D-6734-2013; Rud, Vyacheslav/D-6838-2012; Alexa, Calin/F-6345-2010; Orlov, Ilya/E-6611-2012; Petrucci, Fabrizio/G-8348-2012; Annovi, Alberto/G-6028-2012; Brooks, William/C-8636-2013; Snesarev, Andrey/H-5090-2013; Tomasek, Lukas/G-6370-2014; Svatos, Michal/G-8437-2014; Chudoba, Jiri/G-7737-2014; Peleganchuk, Sergey/J-6722-2014; Santamarina Rios, Cibran/K-4686-2014; Bosman, Martine/J-9917-2014; Lei, Xiaowen/O-4348-2014; Demirkoz, Bilge/C-8179-2014; Gutierrez, Phillip/C-1161-2011; Ventura, Andrea/A-9544-2015; Mitsou, Vasiliki/D-1967-2009; Lee, Jason/B-9701-2014; Robson, Aidan/G-1087-2011; Smirnova, Oxana/A-4401-2013; Fabbri, Laura/H-3442-2012; Villa, Mauro/C-9883-2009; Nemecek, Stanislav/G-5931-2014; Kepka, Oldrich/G-6375-2014; Jakoubek, Tomas/G-8644-2014; Lokajicek, Milos/G-7800-2014; Staroba, Pavel/G-8850-2014; Kupco, Alexander/G-9713-2014; Mikestikova, Marcela/H-1996-2014; Kuday, Sinan/C-8528-2014; Anjos, Nuno/I-3918-2013; Kartvelishvili, Vakhtang/K-2312-2013; Prokoshin, Fedor/E-2795-2012; Dawson, Ian/K-6090-2013; Solfaroli Camillocci, Elena/J-1596-2012; Tudorache, Valentina/D-2743-2012; Marti-Garcia, Salvador/F-3085-2011; Castro, Nuno/D-5260-2011; Wolters, Helmut/M-4154-2013; Warburton, Andreas/N-8028-2013; De, Kaushik/N-1953-2013; Sukharev, Andrey/A-6470-2014; la rotonda, laura/B-4028-2016; Capua, Marcella/A-8549-2015; Tartarelli, Giuseppe Francesco/A-5629-2016; Fassi, Farida/F-3571-2016; Mashinistov, Ruslan/M-8356-2015; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Yang, Haijun/O-1055-2015; Monzani, Simone/D-6328-2017; Grancagnolo, Francesco/K-2857-2015; Korol, Aleksandr/A-6244-2014; Karyukhin, Andrey/J-3904-2014; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Olshevskiy, Alexander/I-1580-2016; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Mora Herrera, Maria Clemencia/L-3893-2016; Maneira, Jose/D-8486-2011; KHODINOV, ALEKSANDR/D-6269-2015; Goncalo, Ricardo/M-3153-2016; Gauzzi, Paolo/D-2615-2009; Camarri, Paolo/M-7979-2015; Gavrilenko, Igor/M-8260-2015; Tikhomirov, Vladimir/M-6194-2015; Chekulaev, Sergey/O-1145-2015; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; Carvalho, Joao/M-4060-2013; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Wemans, Andre/A-6738-2012; Leyton, Michael/G-2214-2016; Joergensen, Morten/E-6847-2015; Mir, Lluisa-Maria/G-7212-2015; Riu, Imma/L-7385-2014; Cabrera Urban, Susana/H-1376-2015; Garcia, Jose /H-6339-2015; Della Pietra, Massimo/J-5008-2012; Cavalli-Sforza, Matteo/H-7102-2015; Negrini, Matteo/C-8906-2014; Ferrer, Antonio/H-2942-2015; Hansen, John/B-9058-2015; Grancagnolo, Sergio/J-3957-2015; spagnolo, stefania/A-6359-2012; Shmeleva, Alevtina/M-6199-2015 OI Livan, Michele/0000-0002-5877-0062; Vanyashin, Aleksandr/0000-0002-0367-5666; Ferrando, James/0000-0002-1007-7816; La Rosa, Alessandro/0000-0001-6291-2142; Moraes, Arthur/0000-0002-5157-5686; Smirnov, Sergei/0000-0002-6778-073X; Conde Muino, Patricia/0000-0002-9187-7478; Andreazza, Attilio/0000-0001-5161-5759; Boyko, Igor/0000-0002-3355-4662; Kuleshov, Sergey/0000-0002-3065-326X; Stoicea, Gabriel/0000-0002-7511-4614; Doyle, Anthony/0000-0001-6322-6195; Pina, Joao /0000-0001-8959-5044; Moorhead, Gareth/0000-0002-9299-9549; Orlov, Ilya/0000-0003-4073-0326; Petrucci, Fabrizio/0000-0002-5278-2206; Annovi, Alberto/0000-0002-4649-4398; Brooks, William/0000-0001-6161-3570; Tomasek, Lukas/0000-0002-5224-1936; Svatos, Michal/0000-0002-7199-3383; Peleganchuk, Sergey/0000-0003-0907-7592; Santamarina Rios, Cibran/0000-0002-9810-1816; Bosman, Martine/0000-0002-7290-643X; Lei, Xiaowen/0000-0002-2564-8351; Ventura, Andrea/0000-0002-3368-3413; Mitsou, Vasiliki/0000-0002-1533-8886; Lee, Jason/0000-0002-2153-1519; Smirnova, Oxana/0000-0003-2517-531X; Fabbri, Laura/0000-0002-4002-8353; Villa, Mauro/0000-0002-9181-8048; Mikestikova, Marcela/0000-0003-1277-2596; Kuday, Sinan/0000-0002-0116-5494; Prokoshin, Fedor/0000-0001-6389-5399; Solfaroli Camillocci, Elena/0000-0002-5347-7764; Castro, Nuno/0000-0001-8491-4376; Wolters, Helmut/0000-0002-9588-1773; Warburton, Andreas/0000-0002-2298-7315; De, Kaushik/0000-0002-5647-4489; la rotonda, laura/0000-0002-6780-5829; Osculati, Bianca Maria/0000-0002-7246-060X; Amorim, Antonio/0000-0003-0638-2321; Santos, Helena/0000-0003-1710-9291; Coccaro, Andrea/0000-0003-2368-4559; Anjos, Nuno/0000-0002-0018-0633; Smestad, Lillian/0000-0002-0244-8736; Giordani, Mario/0000-0002-0792-6039; Abdelalim, Ahmed Ali/0000-0002-2056-7894; Capua, Marcella/0000-0002-2443-6525; Di Micco, Biagio/0000-0002-4067-1592; Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; Doria, Alessandra/0000-0002-5381-2649; Veloso, Filipe/0000-0002-5956-4244; Gomes, Agostinho/0000-0002-5940-9893; Fassi, Farida/0000-0002-6423-7213; Mashinistov, Ruslan/0000-0001-7925-4676; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Monzani, Simone/0000-0002-0479-2207; Grancagnolo, Francesco/0000-0002-9367-3380; Korol, Aleksandr/0000-0001-8448-218X; Maio, Amelia/0000-0001-9099-0009; Fiolhais, Miguel/0000-0001-9035-0335; Karyukhin, Andrey/0000-0001-9087-4315; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Olshevskiy, Alexander/0000-0002-8902-1793; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Maneira, Jose/0000-0002-3222-2738; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Goncalo, Ricardo/0000-0002-3826-3442; Gauzzi, Paolo/0000-0003-4841-5822; Camarri, Paolo/0000-0002-5732-5645; Tikhomirov, Vladimir/0000-0002-9634-0581; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; Carvalho, Joao/0000-0002-3015-7821; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Wemans, Andre/0000-0002-9669-9500; Leyton, Michael/0000-0002-0727-8107; Joergensen, Morten/0000-0002-6790-9361; Mir, Lluisa-Maria/0000-0002-4276-715X; Riu, Imma/0000-0002-3742-4582; Della Pietra, Massimo/0000-0003-4446-3368; Negrini, Matteo/0000-0003-0101-6963; Ferrer, Antonio/0000-0003-0532-711X; Hansen, John/0000-0002-8422-5543; Grancagnolo, Sergio/0000-0001-8490-8304; spagnolo, stefania/0000-0001-7482-6348; FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union; ERC, European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; ISF, Israel; MINERVA, Israel; GIF, Israel; DIP, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; GRICES, Portugal; FCT, Portugal; MERYS (MECTS), Romania; MES of Russia, Russian Federation; ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MVZT, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET and ERC, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT, Greece; ISF, MINERVA, GIF, DIP and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW, Poland; GRICES and FCT, Portugal; MERYS (MECTS), Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MVZT, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. NR 35 TC 2 Z9 2 U1 7 U2 133 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JAN PY 2013 IS 1 AR 131 DI 10.1007/JHEP01(2013)131 PG 34 WC Physics, Particles & Fields SC Physics GA 098XY UT WOS:000315583600050 ER PT J AU Aad, G Abajyan, T Abbott, B Abdallah, J Khalek, SA Abdelalim, AA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Acharya, BS Adamczyk, L Adams, DL Addy, TN Adelman, J Adomeit, S Adragna, P Adye, T Aefsky, S Aguilar-Saavedra, JA Agustoni, M Aharrouche, M Ahlen, SP Ahles, F Ahmad, A Ahsan, M Aielli, G Akesson, TPA Akimoto, G Akimov, AV Alam, MS Alam, MA Albert, J Albrand, S Aleksa, M Aleksandrov, IN Alessandria, F Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Aliev, M Alimonti, G Alison, J Allbrooke, BMM Allport, PP Allwood-Spiers, SE Almond, J Aloisio, A Alon, R Alonso, A Alonso, F Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Amelung, C Ammosov, VV Dos Santos, SPA Amorim, A Amram, N Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Andrieux, ML 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JBG Bartoldus, R Barton, AE Bartsch, V Basye, A Bates, RL Batkova, L Batley, JR Battaglia, A Battistin, M Bauer, F Bawa, HS Beale, S Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, S Beckingham, M Becks, KH Beddall, AJ Beddall, A Bedikian, S Bednyakov, VA Bee, CP Beemster, LJ Begel, M Harpaz, SB Behera, PK Beimforde, M Belanger-Champagne, C Bell, PJ Bell, WH Bella, G Bellagamba, L Bellomo, M Belloni, A Beloborodova, O Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Benoit, M Bensinger, JR Benslama, K Bentvelsen, S Berge, D Kuutmann, EB Berger, N Berghaus, F Berglund, E Beringer, J Bernat, P Bernhard, R Bernius, C Berry, T Bertella, C Bertin, A Bertolucci, F Besana, MI Besjes, GJ Besson, N Bethke, S Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Bieniek, SP Bierwagen, K Biesiada, J Biglietti, M Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Biscarat, C Bittner, B Black, CW 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CA ATLAS Collaboration TI Measurement of isolated-photon pair production in pp collisions at root s=7 TeV with the ATLAS detector SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering ID PARTON DISTRIBUTIONS; BOSON; LHC; HIERARCHY; MASS AB The ATLAS experiment at the LHC has measured the production cross section of events with two isolated photons in the final state, in proton-proton collisions at root s = 7 TeV. The full data set collected in 2011, corresponding to an integrated luminosity of 4.9 fb(-1), is used. The amount of background, from hadronic jets and isolated electrons, is estimated with data-driven techniques and subtracted. The total cross section, for two isolated photons with transverse energies above 25 GeV and 22 GeV respectively, in the acceptance of the electromagnetic calorimeter (vertical bar eta vertical bar < 1.37 and 1.52 < vertical bar eta vertical bar 2.37) and with an angular separation Delta R > 0.4, is 44.0(-4.2)(+3.2) pb. The differential cross sections as a function of the di-photon invariant mass, transverse momentum, azimuthal separation, and cosine of the polar angle of the largest transverse energy photon in the Collins-Soper di-photon rest frame are also measured. The results are compared to the prediction of leading-order parton-shower and next-to-leading-order and next-to-next-to-leading-order parton-level generators. C1 [Jackson, P.; Soni, N.] Univ Adelaide, Sch Chem & Phys, Adelaide, SA, Australia. [Alam, M. S.; Edson, W.; Ernst, J.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Bahinipati, S.; Chan, K.; Gingrich, D. M.; Moore, R. W.; Pinfold, J. L.; Subramania, H. S.; Vaque, F. Vives] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakir, O.; Ciftci, A. K.; Ciftci, R.; Yildiz, H. Duran; Kuday, S.] Ankara Univ, Dept Phys, TR-06100 Ankara, Turkey. Dumlupinar Univ, Dept Phys, Kutahya, Turkey. [Yilmaz, M.] Gazi Univ, Dept Phys, Ankara, Turkey. 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G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Anastopoulos, C.; Anghinolfi, F.; Avolio, G.; Baak, M. A.; Banfi, D.; Battistin, M.; Bellomo, M.; Beltramello, O.; Berge, D.; Bianchi, R. M.; Blanchot, G.; Bogaerts, J. A.; Boyd, J.; Bremer, J.; Burckhart, H.; Byszewski, M.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Catmore, J. R.; Cattai, A.; Barajas, C. A. Chavez; Childers, J. T.; Chromek-Burckhart, D.; Cote, D.; Danielsson, H. O.; Dell'Acqua, A.; Di Girolamo, A.; Di Girolamo, B.; Di Micco, B.; Dittus, F.; Dobos, D.; Dobson, E.; Dopke, J.; Dudarev, A.; Uhrssen, M. D.; Ellis, N.; Elsing, M.; Fabre, C.; Farthouat, P.; Fassnacht, P.; Francis, D.; Franz, S.; Froidevaux, D.; Gabaldon, C.; Garelli, N.; Garonne, V.; Gianotti, F.; Gibson, S. M.; Godlewski, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Haas, S.; Hahn, F.; Hauschild, M.; Hawkings, R. J.; Heller, M.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Huhtinen, M.; Jaekel, M. R.; Jansen, H.; Jenni, P.; Joram, C.; Jungst, R. M.; Kaneda, M.; Kaplon, J.; Kerschen, N.; Klioutchnikova, T.; Koeneke, K.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malaescu, B.; Malyukov, S.; Mapelli, A.; Mapelli, L.; Marshall, Z.; Martin, B.; Messina, A.; Michal, S.; Molfetas, A.; Morley, A. K.; Mornacchi, G.; Muenstermann, D.; Nairz, A. M.; Nakahama, Y.; Negri, G.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Ohm, C. C.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Petersen, J.; Piacquadio, G.; Pommes, K.; Poppleton, A.; Bueso, X. Portell; Poulard, G.; Prasad, S.; Raymond, M.; Rembser, C.; Dos Santos, D. Roda; Roe, S.; Salek, D.; Salzburger, A.; Savu, D. O.; Schlenker, S.; Schott, M.; Sfyrla, A.; Spigo, G.; Spiwoks, R.; Stewart, G. A.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van der Ster, D.; van Eldik, N.; Vandelli, W.; Veness, R.; Vinek, E.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Winklmeier, F.; Wotschack, J.; Zwalinski, L.] CERN, Geneva, Switzerland. [Anderson, K. J.; Boveia, A.; Canelli, F.; Cheng, Y.; Choudalakis, G.; Fiascaris, M.; Gardner, R. W.; Plante, I. Jen-La; Kapliy, A.; Li, H. L.; Meehan, S.; Melachrinos, C.; Merritt, F. S.; Meyer, C.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Shochet, M. J.; Tompkins, L.; Tuggle, J. M.; Vukotic, I.; Webster, J. S.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Diaz, M. A.; Olivares Pino, S. A.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Carquin, E.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lu, F.; Ouyang, Q.; Ruan, X.; Shan, L. Y.; Wang, J.; Xu, D.; Yao, L.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Han, L.; Jiang, Y.; Li, B.; Li, S.; Liu, M.; Liu, Y.; Peng, H.; Wu, Y.; Xu, C.; Xu, L.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Feng, C.; Ge, P.; Meng, Z.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Tsinan, Shandong, Peoples R China. Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200030, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Toro, R. Camacho; Cinca, D.; Donini, J.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Vazeille, F.] Univ Clermont Ferrand, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Toro, R. Camacho; Cinca, D.; Donini, J.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Toro, R. Camacho; Cinca, D.; Donini, J.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Vazeille, F.] CNRS IN2P3, Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Brooijmans, G.; Chen, Y.; Dodd, J.; Grau, N.; Guo, J.; Hu, D.; Hughes, E. W.; Nikiforou, N.; Parsons, J. A.; Penson, A.; Perez, K.; Reale, V. Perez; Scherzer, M. I.; Spousta, M.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Williams, E.; Willis, W.; Wulf, E.; Zivkovic, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Boelaert, N.; Dam, M.; Gregersen, K.; Hansen, J. R.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Heisterkamp, S.; Jakobsen, S.; Loevschall-Jensen, A. E.; Jez, P.; Joergensen, M. D.; Kadlecik, P.; Klinkby, E. B.; Lundquist, J.; Mackeprang, R.; Mehlhase, S.; Petersen, T. C.; Pingel, A.; Simonyan, M.; Thomsen, L. A.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; Fazio, S.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Morello, G.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Grp Coll Cosenza, Arcavacata Di Rende, Italy. [Capua, M.; Crosetti, G.; Fazio, S.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Morello, G.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Banas, E.; Blocki, J.; de Renstrom, P. A. Bruckman; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Malecki, P.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Turala, M.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.; Zemla, A.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Yagci, K. Dindar; Firan, A.; Hoffman, J.; Joffe, D.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Rios, R. R.; Sekula, S. J.; Stroynowski, R.; Wang, H.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Ahsan, M.; Izen, J. M.; Lou, X.; Reeves, K.; Wong, W. C.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Kuutmann, E. Bergeaas; Bloch, I.; Dassoulas, J. A.; Dietrich, J.; Ehrenfeld, W.; Ferrara, V.; Fischer, G.; Friedrich, C.; Glazov, A.; Goebel, M.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K-J.; Gregor, I. M.; Hiller, K. H.; Huettmann, A.; Belenguer, M. Jimenez; Johnert, S.; Katzy, J.; Kono, T.; Kuhl, T.; Lange, C.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Cavalcanti, T. Perez; Petschull, D.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Zhu, H.] DESY, Hamburg, Germany. [Argyropoulos, S.; Kuutmann, E. Bergeaas; Bloch, I.; Dassoulas, J. A.; Dietrich, J.; Ehrenfeld, W.; Ferrara, V.; Fischer, G.; Friedrich, C.; Glazov, A.; Goebel, M.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K-J.; Gregor, I. M.; Hiller, K. H.; Huettmann, A.; Belenguer, M. Jimenez; Johnert, S.; Katzy, J.; Kono, T.; Kuhl, T.; Lange, C.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Cavalcanti, T. Perez; Petschull, D.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Zhu, H.] DESY, Zeuthen, Germany. [Bunse, M.; Esch, H.; Goessling, C.; Hirsch, F.; Jung, C. A.; Klingenberg, R.; Reisinger, I.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Czodrowski, P.; Friedrich, F.; Goepfert, T.; Kobel, M.; Leonhardt, K.; Ludwig, A.; Mader, W. F.; Morgenstern, M.; Prudent, X.; Rudolph, C.; Schnoor, U.; Schwierz, R.; Seifert, F.; Steinbach, P.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Ebenstein, W. L.; Fowler, A. J.; Ko, B. R.; Kotwal, A.; Kruse, M. K.; Oh, S. H.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Buckley, A. G.; Clark, P. J.; Debenedetti, C.; Harrington, R. D.; Martin, V. J.; O'Brien, B. J.; Schaelicke, A.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.; Volpi, G.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Aad, G.; Ahles, F.; Barber, T.; Bernhard, R.; Boehler, M.; Bruneliere, R.; Christov, A.; Consorti, V.; Fehling-Kaschek, M.; Flechl, M.; Hartert, J.; Herten, G.; Horner, S.; Jakobs, K.; Janus, M.; Kononov, A. I.; Kuehn, S.; Lai, S.; Landgraf, U.; Lohwasser, K.; Ludwig, I.; Ludwig, J.; Mahboubi, K.; Mohr, W.; Nilsen, H.; Parzefall, U.; Rammensee, M.; Rave, T. C.; Rurikova, Z.; Schmidt, E.; Schumacher, M.; Siegert, F.; Stoerig, K.; Sundermann, J. E.; Temming, K. K.; Thoma, S.; Tsiskaridze, V.; Venturi, M.; Vivarelli, I.; von Radziewski, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Winkelmann, S.; Xie, S.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Abdelalim, A. A.; Alexandre, G.; Backes, M.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; Blondel, A.; Bucci, F.; Clark, A.; Dao, V.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Iacobucci, G.; La Rosa, A.; Lister, A.; Latour, B. Martin Dit; Mermod, P.; Herrera, C. Mora; Nektarijevic, S.; Nessi, M.; Nikolics, K.; Pasztor, G.; Picazio, A.; Pohl, M.; Rosbach, K.; Rosselet, L.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Beccherle, R.; Caso, C.; Dameri, M.; Darbo, G.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Barberis, D.; Caso, C.; Dameri, M.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Chikovani, L.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Khubua, J.; Mchedlidze, G.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Bussey, P.; Buttar, C. M.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Edwards, N. C.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Kar, D.; Kenyon, M.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Saxon, D. H.; Smith, K. M.; St Denis, R. D.; Steele, G.; Thompson, A. S.; Wraight, K.; Wright, M.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bierwagen, K.; Blumenschein, U.; Brandt, O.; Evangelakou, D.; George, M.; Grosse-Knetter, J.; Guindon, S.; Hamer, M.; Hensel, C.; Keil, M.; Knue, A.; Kohn, F.; Krieger, N.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Meyer, J.; Morel, J.; Nackenhorst, O.; Pashapour, S.; Quadt, A.; Roe, A.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Uhrmacher, M.; Schroeder, T. Vazquez; Weingarten, J.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Andrieux, M-L.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Stark, J.; Sun, X.; Trocme, B.; Weydert, C.] Univ Grenoble 1, Lab Phys Subatom & Cosmol, Grenoble, France. [Albrand, S.; Andrieux, M-L.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Stark, J.; Sun, X.; Trocme, B.; Weydert, C.] CNRS IN2P3, Grenoble, France. [Albrand, S.; Andrieux, M-L.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Stark, J.; Sun, X.; Trocme, B.; Weydert, C.] Inst Natl Polytech Grenoble, F-38031 Grenoble, France. [Addy, T. N.; Harvey, A.; McFarlane, K. W.; Shin, T.; Vassilakopoulos, V. I.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Belloni, A.; Catastini, P.; Conti, G.; Franklin, M.; Huth, J.; Jeanty, L.; Kagan, M.; Mateos, D. Lopez; Outschoorn, V. Martinez; Mercurio, K. M.; Mills, C.; Morii, M.; Skottowe, H. P.; Smith, B. C.; Yen, A. L.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Anders, G.; Andrei, V.; Davygora, Y.; Dietzsch, T. A.; Dunford, M.; Geweniger, C.; Hanke, P.; Henke, M.; Khomich, A.; Kluge, E. -E.; Lang, V. S.; Lendermann, V.; Lepold, F.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Karnevskiy, M.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Kugel, A.; Maenner, R.; Schroer, N.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Cwetanski, P.; Evans, H.; Gagnon, P.; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Price, D.; Whittington, D.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Epp, B.; Jussel, P.; Kneringer, E.; Kuhn, D.; Lukas, W.; Rudolph, G.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Behera, P. K.; Limper, M.; Mallik, U.; Mandrysch, R.; Pylypchenko, Y.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Rosenberg, E. I.; Ruiz-Martinez, A.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Aleksandrov, I. N.; Bardin, D. Y.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Grigalashvili, N.; Huseynov, N.; Kalinovskaya, L. V.; Kazarinov, M. Y.; Kekelidze, G. D.; Kharchenko, D.; Khramov, E.; Kolesnikov, V.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Pozdnyakov, V.; Rumyantsev, L.; Rusakovich, N. A.; Sadykov, R.; Shiyakova, M.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.; Zimin, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Arai, Y.; Doi, Y.; Haruyama, T.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Makida, Y.; Manabe, A.; Mitsui, S.; Nagano, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Hayakawa, T.; King, M.; Kishimoto, T.; Kitamura, T.; Kurashige, H.; Matsushita, T.; Ochi, A.; Suzuki, Y.; Takeda, H.; Tani, K.; Watanabe, I.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Sasao, N.; Sumida, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.; Ventura, A.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.; Ventura, A.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Davidson, R.; de Mora, L.; Dearnaley, W. J.; Fox, H.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Bianco, M.; Cataldi, G.; Chiodini, G.; Gorini, E.; Grancagnolo, F.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Bianco, M.; Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Greenshaw, T.; Gwilliam, C. B.; Hayward, H. S.; Jackson, J. N.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kluge, T.; Kretzschmar, J.; Laycock, P.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Sellers, G.; Vossebeld, J. H.; Waller, P.; Wrona, B.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia. [Adragna, P.; Bona, M.; Carter, A. A.; Cerrito, L.; Eisenhandler, E.; Ellis, K.; Goddard, J. R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Poll, J.; Rizvi, E.; Salamanna, G.; Castanheira, M. Teixeira Dias; Wiglesworth, C.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Alam, M. A.; Berry, T.; Boisvert, V.; Brooks, T.; Cantrill, R.; Cowan, G.; Duguid, L.; Edwards, C. A.; George, S.; Goncalo, R.; Hayden, D.; Vazquez, J. G. Panduro; Pastore, Fr.; Rose, M.; Spano, F.; Strong, J. A.; Teixeira-Dias, P.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Baker, S.; Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Chislett, R. T.; Christidi, I. A.; Cooper, B. D.; Davison, A. R.; Dobson, E.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Lambourne, L.; Monk, J.; Nash, M.; Nurse, E.; Prabhu, R.; Sherwood, P.; Simmons, B.; Taylor, C.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Cavalleri, P.; Crescioli, F.; Davignon, O.; De Cecco, S.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph.; Theveneaux-Pelzer, T.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Cavalleri, P.; Crescioli, F.; Davignon, O.; De Cecco, S.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph.; Theveneaux-Pelzer, T.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Cavalleri, P.; Crescioli, F.; Davignon, O.; De Cecco, S.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph.; Theveneaux-Pelzer, T.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] CNRS IN2P3, Paris, France. [Akesson, T. P. A.; Alonso, A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Jarlskog, G.; Lundberg, B.; Lytken, E.; Meirose, B.; Mjornmark, J. U.; Smirnova, O.] Lund Univ, Fysiska Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Labarga, L.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Aharrouche, M.; Arnaez, O.; Blum, W.; Uscher, V. B.; Caputo, R.; Eckweiler, S.; Edmonds, K.; Ellinghaus, F.; Ertel, E.; Fiedler, F.; Fleckner, J.; Goeringer, C.; Handel, C.; Hohlfeld, M.; Hsu, P. J.; Ji, W.; Kawamura, G.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lungwitz, M.; Masetti, L.; Meyer, C.; Moreno, D.; Mueller, T.; Neusiedl, A.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schroeder, C.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Almond, J.; Borri, M.; Brown, G.; Chavda, V.; Cox, B. E.; Da Via, C.; Duerdoth, I. P.; Forti, A.; Howarth, J.; Ibbotson, M.; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Marx, M.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Pilkington, A. D.; Robinson, J. E. M.; Snow, S. W.; Watts, S.; Woudstra, M. J.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aoun, S.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Li, S.; Maurer, J.; Monnier, E.; Odier, J.; Pralavorio, P.; Rozanov, A.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aoun, S.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Li, S.; Maurer, J.; Monnier, E.; Odier, J.; Pralavorio, P.; Rozanov, A.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] CNRS IN2P3, Marseille, France. [Brau, B.; Colon, G.; Dallapiccola, C.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Caron, B.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Dobbs, M.; Dufour, M-A.; Klemetti, M.; Mc Donald, J.; Robertson, S. H.; Rios, C. Santamarina; Schram, M.; Stockton, M. C.; Vachon, B.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Davidson, N.; Diglio, S.; Hamano, K.; Jennens, D.; Kubota, T.; Limosani, A.; Moorhead, G. F.; Hanninger, G. Nunes; Phan, A.; Shao, Q. T.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Volpi, M.; White, M. J.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Armbruster, A. J.; Borroni, S.; Chapman, J. W.; Cirilli, M.; Dai, T.; Diehl, E. B.; Ferretti, C.; Goldfarb, S.; Harper, D.; Levin, D.; Li, X.; Liu, J. B.; Liu, L.; Mc Kee, S. P.; Neal, H. A.; Panikashvili, N.; Purdham, J.; Qian, J.; Scheirich, D.; Thun, R. P.; Walch, S.; Wilson, A.; Wooden, G.; Wu, Y.; Yang, H.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Fedorko, W.; Hauser, R.; Holzbauer, J. L.; Huston, J.; Koll, J.; Linnemann, J. T.; Martin, B.; Miller, R. J.; Pope, B. G.; Schwienhorst, R.; Stelzer, H. J.; Tollefson, K.; True, P.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alessandria, F.; Alimonti, G.; Andreazza, A.; Baccaglioni, G.; Besana, M. I.; Broggi, F.; Carminati, L.; Cavalli, D.; Citterio, M.; Consonni, S. M.; Costa, G.; Fanti, M.; Favareto, A.; Giugni, D.; Koletsou, I.; Lari, T.; Mandelli, L.; Mazzanti, M.; Meloni, F.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Rivoltella, G.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Vegni, G.; Volpini, G.] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Andreazza, A.; Besana, M. I.; Carminati, L.; Consonni, S. M.; Fanti, M.; Favareto, A.; Meloni, F.; Perini, L.; Pizio, C.; Ragusa, F.; Rivoltella, G.; Simoniello, R.; Turra, R.; Vegni, G.] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Satsounkevitch, I.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Banerjee, P.; Bouchami, J.; Dallaire, F.; Davies, M.; Giunta, M.; Leroy, C.; Martin, J. P.; Soueid, P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.] Acad Sci, PN Lebedev Inst Phys, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.] Moscow Engn & Phys Inst, Moscow, Russia. [Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Beale, S.; Becker, S.; Biebel, O.; Bortfeldt, J.; Calfayan, P.; de Graat, J.; Duckeck, G.; Ebke, J.; Elmsheuser, J.; Engl, A.; Galea, C.; Heller, C.; Hertenberger, R.; Kummer, C.; Legger, F.; Lichtnecker, M.; Lorenz, J.; Mann, A.; Mueller, T. A.; Nunnemann, T.; Oakes, L. B.; Rauscher, F.; Reznicek, P.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Schieck, J.; Serfon, C.; Staude, A.; Vladoiu, D.; Walker, R.; Will, J. Z.; Zhuang, X.; Zibell, A.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Beimforde, M.; Bethke, S.; Bittner, B.; Bronner, J.; Capriotti, D.; Compostella, G.; Cortiana, G.; Dubbert, J.; Flowerdew, M. J.; Giovannini, P.; Ince, T.; Jantsch, A.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kotov, S.; Kroha, H.; Macchiolo, A.; Manfredini, A.; Menke, S.; Moser, H. G.; Nagel, M.; Nisius, R.; Oberlack, H.; Pahl, C.; Pospelov, G. E.; Potrap, I. N.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Stern, S.; Stonjek, S.; Vanadia, M.; von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.; Zhuravlov, V.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Shimizu, S.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Shimizu, S.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Capasso, L.; Carlino, G.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; della Volpe, D.; Di Donato, C.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Patricelli, S.; Sanchez, A.; Sekhniaidze, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Capasso, L.; Chiefari, G.; della Volpe, D.; Di Donato, C.; Giordano, R.; Merola, L.; Patricelli, S.; Sanchez, A.] Univ Naples Federico II, Dipartimento Sci Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Chelstowska, M. A.; De Groot, N.; Filthaut, F.; Klok, P. F.; Konig, A. C.; Koetsveld, F.; Raas, M.; Salvucci, A.] Radboud Univ Nijmegen, Nikhef, Inst Math Astrophys & Particle Phys, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Doxiadis, A. D.; Ferrari, P.; Garitaonandia, H.; Geerts, D. A. A.; Gosselink, M.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kayl, M. S.; Klous, S.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Luijckx, G.; Mahlstedt, J.; Massaro, G.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Pani, P.; Rijpstra, M.; Ruckstuhl, N.; Ta, D.; Tsiakiris, M.; Turlay, E.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van der Poel, E.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Doxiadis, A. D.; Ferrari, P.; Garitaonandia, H.; Geerts, D. A. A.; Gosselink, M.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kayl, M. S.; Klous, S.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Luijckx, G.; Mahlstedt, J.; Massaro, G.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Pani, P.; Rijpstra, M.; Ruckstuhl, N.; Ta, D.; Tsiakiris, M.; Turlay, E.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van der Poel, E.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.] Univ Amsterdam, Amsterdam, Netherlands. [Anisenkov, A.; Beloborodova, O.; Bobrovnikov, V. S.; Bogdanchikov, A.; Kazanin, V. F.; Kolachev, G. M.; Korol, A.; Malyshev, V.; Maslennikov, A. L.; Maximov, D. A.; Orlov, I.; Peleganchuk, S. V.; Schamov, A. G.; Skovpen, K.; Soukharev, A.; Talyshev, A.; Tikhonov, Y. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Budick, B.; Casadei, D.; Cranmer, K.; Haas, A.; van Huysduynen, L. Hooft; Kaplan, B.; Konoplich, R.; Krasznahorkay, A.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.; Prokofiev, K.; Zhao, L.] NYU, Dept Phys, New York, NY 10003 USA. [Fisher, M. J.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Rahimi, A. M.; Strang, M.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Gutierrez, P.; Jana, D. K.; Marzin, A.; Meera-Lebbai, R.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Snow, J.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Khanov, A.; Rizatdinova, F.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Hamal, P.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Potter, C. T.; Ptacek, E.; Radloff, P.; Reinsch, A.; Searcy, J.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Andari, N.; Auge, E.; Benoit, M.; Binet, S.; Bourdarios, C.; De la Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Niedercorn, F.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Ruan, X.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Teinturier, M.; Veillet, J. J.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Andari, N.; Auge, E.; Benoit, M.; Binet, S.; Bourdarios, C.; De la Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Niedercorn, F.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Ruan, X.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Teinturier, M.; Veillet, J. J.; Zerwas, D.; Zhang, Z.] CNRS IN2P3, Orsay, France. [Hanagaki, K.; Hirose, M.; Lee, J. S. H.; Meguro, T.; Nomachi, M.; Okamura, W.; Sugaya, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Buran, T.; Cameron, D.; Gjelsten, B. K.; Gramstad, E.; Lund, E.; Ould-Saada, F.; Pajchel, K.; Read, A. L.; Rohne, O.; Samset, B. H.; Smestad, L.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Apolle, R.; Barr, A. J.; Boddy, C. R.; Brandt, G.; Buchanan, J.; Buckingham, R. M.; Cooper-Sarkar, A. M.; Dafinca, A.; Davies, E.; Gallas, E. J.; Gwenlan, C.; Hall, D.; Hays, C. P.; Howard, J.; Huffman, T. B.; Issever, C.; King, R. S. B.; Kogan, L. A.; Korn, A.; Larner, A.; Lewis, A.; Liang, Z.; Livermore, S. S. A.; Mattravers, C.; Nickerson, R. B.; Pinder, A.; Robichaud-Veronneau, A.; Ryder, N. C.; Short, D.; Tseng, J. C-L.; Vickey, T.; Viehhauser, G. H. A.; Weidberg, A. R.; Whitehead, S. R.; Young, C. J.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Colombo, T.; Conta, C.; Ferrari, R.; Franchino, S.; Fraternali, M.; Gaudio, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Uslenghi, M.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Colombo, T.; Conta, C.; Franchino, S.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.; Uslenghi, M.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Alison, J.; Brendlinger, K.; Degenhardt, J.; Dressnandt, N.; Fratina, S.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Keener, P. T.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Newcomer, F. M.; Olivito, D.; Ospanov, R.; Reece, R.; Saxon, J.; Schaefer, D.; Stahlman, J.; Thomson, E.; Van Berg, R.; Wagner, P.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Bertolucci, F.; Cascella, M.; Cavasinni, V.; Del Prete, T.; Dotti, A.; Roda, C.; Sarri, F.; White, S.; Zinonos, Z.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Bertolucci, F.; Cascella, M.; Cavasinni, V.; Del Prete, T.; Dotti, A.; Roda, C.; Sarri, F.; White, S.; Zinonos, Z.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Boudreau, J.; Cleland, W.; Escobar, C.; Kittelmann, T.; Mueller, J.; Prieur, D.; Savinov, V.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Anjos, N.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Do Valle Wemans, A.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Jorge, P. M.; Lopes, L.; Machado Miguens, J.; Maio, A.; Maneira, J.; Oliveira, M.; Onofre, A.; Palma, A.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. [Bohm, J.; Chudoba, J.; Gallus, P.; Gunther, J.; Jakoubek, T.; Juranek, V.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Marcisovsky, M.; Mikestikova, M.; Myska, M.; Nemecek, S.; Ruzicka, P.; Schovancova, J.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Tic, T.; Valenta, J.; Vrba, V.; Zeman, M.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Holy, T.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Kral, V.; Krejci, F.; Pospisil, S.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solar, M.; Solc, J.; Sopko, V.; Sopko, B.; Stekl, I.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Torregrosa, E. Fullana; Kodys, P.; Leitner, R.; Novakova, J.; Rybar, M.; Spousta, M.; Strachota, P.; Suk, M.; Sykora, T.; Tas, P.; Valkar, S.; Vorobel, V.; Wilhelm, I.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Ammosov, V. V.; Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Ivashin, A. V.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.; Zmouchko, V. V.] Inst High Energy Phys, State Res Ctr, Protvino, Russia. [Adye, T.; Apolle, R.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Gillman, A. R.; Haywood, S. J.; Kirk, J.; Mattravers, C.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Nash, M.; Norton, P. R.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Benslama, K.] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Artoni, G.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Pedis, D.; De Salvoa, A.; De Zorzi, G.; Dionisi, C.; Falciano, S.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Rossi, E.; Tehrani, F. Safai; Sidoti, A.; Camillocci, E. Solfaroli; Vari, R.; Veneziano, S.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma 1, Rome, Italy. [Artoni, G.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Zorzi, G.; Dionisi, C.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Messina, A.; Rossi, E.; Camillocci, E. Solfaroli; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Di Simone, A.; Liberti, B.; Marchese, F.; Mazzaferro, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Cattani, G.; Di Ciaccio, A.; Di Simone, A.; Marchese, F.; Mazzaferro, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Branchini, P.; Ceradini, F.; Di Luise, S.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Stanescu, C.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Luise, S.; Orestano, D.; Pastore, F.; Petrucci, F.] Univ Roma Tre, Dipartimento Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.; Lablak, S.] Univ Hassan 2, Fac Sci Ain Chock, Reseau Univ Phys Hautes Energies, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA Marrakech, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [Cherkaoui El Moursli, R.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Abreu, H.; Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Bolnet, N. M.; Boonekamp, M.; Chevalier, L.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Gauthier, L.; Giraud, P. F.; Guyot, C.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Legendre, M.; Maiani, C.; Mal, P.; Ramos, J. A. Manjarres; Mansoulie, B.; Meyer, J-P.; Mijovic, L.; Morange, N.; Mountricha, E.; Hong, V. Nguyen Thi; Nicolaidou, R.; Ouraou, A.; Resende, B.; Royon, C. R.; Schoeffel, L.; Schune, Ph.; Schwindling, J.; Simard, O.; Virchaux, M.; Vranjes, N.; Xiao, M.; Xu, C.] CEA Saclay Commissariat Energie Atom, DSM IRFU Inst Rech Lois Fondamentales Univers, Gif Sur Yvette, France. [Chouridou, S.; Damiani, D. S.; Grillo, A. A.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Mitrevski, J.; Nielsen, J.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Beckingham, M.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Hsu, S. -C.; Keller, J. S.; Lubatti, H. J.; Rompotis, N.; Rothberg, J.; Verducci, M.; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Duxfield, R.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Mayne, A.; Mcfayden, J. A.; Miyagawa, P. S.; Owen, S.; Paganis, E.; Suruliz, K.; Tovey, D. R.; Tsionou, D.; Tua, A.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Holder, M.; Ibragimov, I.; Rammes, M.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Dawe, E.; Godfrey, J.; Kvita, J.; O'Neil, D. C.; Petteni, M.; Stelzer, B.; Tanasijczuk, A. J.; Trottier-McDonald, M.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Mayes, J. Backus; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Butler, B.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Grenier, P.; Hansson, P.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nelson, T. K.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Smith, D.; Strauss, E.; Su, D.; Wilson, M. G.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Antos, J.; Batkova, L.; Blazek, T.; Federic, P.; Pecsy, M.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Bruncko, D.; Ferencei, J.; Kladiva, E.; Seman, M.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Assamagan, K.; Aurousseau, M.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Carrillo-Montoya, G. D.; Hamilton, A.; Leney, K. J. C.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Asman, B.; Bendtz, K.; Bohm, C.; Clement, C.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Holmgren, S. O.; Johansen, M.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Papadelis, A.; Sellden, B.; Silverstein, S. B.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Asman, B.; Bendtz, K.; Clement, C.; Gellerstedt, K.; Hellman, S.; Johansen, M.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Ahmad, A.; Arfaoui, S.; Devetak, E.; DeWilde, B.; Engelmann, R.; Farley, J.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Li, H.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Ahmad, A.; Arfaoui, S.; Devetak, E.; DeWilde, B.; Engelmann, R.; Farley, J.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Li, H.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Bartsch, V.; De Santo, A.; Martin-Haugh, S.; Potter, C. J.; Rose, A.; Salvatore, F.; Castillo, I. Santoyo; Sutton, M. R.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Bangert, A.; Black, C. W.; Cuthbert, C.; Patel, N.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Waugh, A. T.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Chu, M. L.; Hou, S.; Jamin, D. O.; Lee, S. C.; Lin, S. C.; Liu, D.; Mazini, R.; Meng, Z.; Ren, Z. L.; Soh, D. A.; Teng, P. K.; Wang, J.; Wang, S. M.; Weng, Z.; Zhou, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Harpaz, S. Behar; Di Mattia, A.; Kajomovitz, E.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; Vallecorsa, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Bella, G.; Benary, O.; Benhammou, Y.; Etzion, E.; Gershon, A.; Ginzburg, J.; Guttman, N.; Hod, N.; Munwes, Y.; Oren, Y.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Iliadis, D.; Kordas, K.; Kouskoura, V.; Nomidis, I.; Petridis, A.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, K.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yamazaki, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, K.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yamazaki, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Ishitsuka, M.; Jinnouchi, O.; Kanno, T.; Kuze, M.; Nagai, R.; Nobe, T.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Bailey, D. C.; Bain, T.; Brelier, B.; Cheung, S. L.; Dhaliwal, S.; Farooque, T.; Fatholahzadeh, B.; Gibson, A.; Guo, B.; Ilic, N.; Keung, J.; Krieger, P.; Orr, R. S.; Rezvani, R.; Rosenbaum, G. A.; Savard, P.; Sinervo, P.; Spreitzer, T.; Tardif, D.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Fortin, D.; Gingrich, D. M.; Koutsman, A.; Losty, M. J.; Nugent, I. M.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Bustos, A. C. Florez; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hanawa, K.; Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Kurata, M.; Nagai, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Napier, A.; Rolli, S.; Sliwa, K.; Todorova-Nova, S.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Loureiro, K. F.; Mendoza Navas, L.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Farrell, S.; Eschrich, I. Gough; Lankford, A. J.; Magnoni, L.; Mete, A. S.; Nelson, A.; Rao, K.; Scannicchio, D. A.; Schernau, M.; Taffard, A.; Toggerson, B.; Unel, G.; Werth, M.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Pinamonti, M.; Shaw, K.; Soualah, R.] Ist Nazl Fis Nucl, Grp Coll Udine, Udine, Italy. [Acharya, B. S.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Giordani, M. P.; Pinamonti, M.; Shaw, K.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Coggeshall, J.; Cortes-Gonzalez, A.; Errede, D.; Errede, S.; Lie, K.; Liss, T. M.; McCarn, A.; Neubauer, M. S.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Brenner, R.; Buszello, C. P.; Coniavitis, E.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Pelikan, D.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] CSIC, Valencia, Spain. [Axen, D.; Gay, C.; Gecse, Z.; Loh, C. W.; Mills, W. J.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Astbury, A.; Bansal, V.; Berghaus, F.; Courneyea, L.; Fincke-Keeler, M.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Lessard, J-R.; Marino, C. P.; Martyniuk, A. C.; McPherson, R. A.; Ouellette, E. A.; Sobie, R.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Farrington, S. M.; Jones, G.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Kimura, N.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Alon, R.; Barak, L.; Bressler, S.; Citron, Z. H.; Duchovni, E.; Frank, T.; Gabizon, O.; Gross, E.; Groth-Jensen, J.; Klier, A.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Milstein, D.; Roth, I.; Silbert, O.; Smakhtin, V.; Vitells, O.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Castaneda Hernandez, A. M.; Castaneda-Miranda, E.; Chen, X.; Dos Anjos, A.; Castillo, L. R. Flores; Gutzwiller, O.; Jared, R. C.; Ji, H.; Ju, X.; Kashif, L.; Ma, L. L.; Garcia, B. R. Mellado; Ming, Y.; Pan, Y. B.; Morales, M. I. Pedraza; Quayle, W. B.; Sarangi, T.; Wang, H.; Wiedenmann, W.; Wu, S. L.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Fleischmann, P.; Meyer, J.; Redelbach, A.; Siragusa, G.; Stroehmer, R.; Trefzger, T.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Barisonzi, M.; Becker, K.; Becks, K. H.; Boek, J.; Boek, T. T.; Braun, H. M.; Cornelissen, T.; Duda, D.; Fleischmann, S.; Flick, T.; Gerlach, P.; Glitza, K. W.; Gorfine, G.; Hamacher, K.; Harenberg, T.; Hirschbuehl, D.; Kalinin, S.; Kersten, S.; Khoroshilov, A.; Kohlmann, S.; Lantzsch, K.; Lenzen, G.; Maettig, P.; Mechtel, M.; Neumann, M.; Pataraia, S.; Sandhoff, M.; Sartisohn, G.; Schultes, J.; Sturm, P.; Wagner, W.; Wahlen, H.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany. [Adelman, J.; Baker, O. K.; Bedikian, S.; Almenar, C. Cuenca; Cummings, J.; Czyczula, Z.; Demers, S.; Erdmann, J.; Garberson, F.; Golling, T.; Guest, D.; Henrichs, A.; Lagouri, T.; Lee, L.; Leister, A. G.; Loginov, A.; Sherman, D.; Tipton, P.; Wall, R.; Walsh, B.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Biscarat, C.; Rahal, G.] Inst Natl Phys Nucl & Phys Particules IN2P3, Ctr Calcul, Villeurbanne, France. [Acharya, B. S.] Kings Coll London, Dept Phys, London WC2R 2LS, England. [Amorim, A.; Gomes, A.; Maio, A.; Pina, J.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amorim, A.; Gomes, A.; Maio, A.; Pina, J.] Univ Lisbon, CFNUL, P-1699 Lisbon, Portugal. [Bawa, H. S.; Gao, Y. S.; Lowe, A. J.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beloborodova, O.; Maximov, D. A.; Talyshev, A.; Tikhonov, Y. A.] Novosibirsk State Univ, Novosiltirsk, Russia. [Carvalho, J.; Fiolhais, M. C. N.; Oliveira, M.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Castaneda Hernandez, A. M.] UASLP, Dept Phys, San Luis Potosi, Mexico. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Demirkoz, B.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Dhullipudi, R.; Greenwood, Z. D.; Sawyer, L.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Do Valle Wemans, A.] Univ Nova Lisboa, Dep Fis, Caparica, Portugal. [Do Valle Wemans, A.] Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, Caparica, Portugal. [Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Kono, T.; Wildt, M. A.] Univ Hamburg, Inst Expt Phys, Hamburg, Germany. [Carvalho, J.; Fiolhais, M. C. N.; Oliveira, M.; Wolters, H.] Manhattan Coll, New York, NY USA. [Liang, Z.; Soh, D. A.; Weng, Z.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou, Peoples R China. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Park, W.; Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Pasztor, G.; Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Perez, K.] CALTECH, Pasadena, CA 91125 USA. [Richter-Was, E.] Jagiellonian Univ, Inst Phys, Krakow, Poland. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. RP Aad, G (reprint author), Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. RI Amorim, Antonio/C-8460-2013; Vanyashin, Aleksandr/H-7796-2013; Ferrando, James/A-9192-2012; Casadei, Diego/I-1785-2013; La Rosa, Alessandro/I-1856-2013; Moraes, Arthur/F-6478-2010; Smirnov, Sergei/F-1014-2011; Conde Muino, Patricia/F-7696-2011; Andreazza, Attilio/E-5642-2011; Boyko, Igor/J-3659-2013; Kuleshov, Sergey/D-9940-2013; Anjos, Nuno/I-3918-2013; Pina, Joao /C-4391-2012; Moorhead, Gareth/B-6634-2009; Ma, Hong/F-2725-2011; Gordon, Howard/D-6734-2013; Rud, Vyacheslav/D-6838-2012; Alexa, Calin/F-6345-2010; Orlov, Ilya/E-6611-2012; Petrucci, Fabrizio/G-8348-2012; Annovi, Alberto/G-6028-2012; Brooks, William/C-8636-2013; Stoicea, Gabriel/B-6717-2011; Fazio, Salvatore /G-5156-2010; Doyle, Anthony/C-5889-2009; Capua, Marcella/A-8549-2015; Tartarelli, Giuseppe Francesco/A-5629-2016; Fassi, Farida/F-3571-2016; la rotonda, laura/B-4028-2016; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Yang, Haijun/O-1055-2015; Monzani, Simone/D-6328-2017; Grancagnolo, Francesco/K-2857-2015; Korol, Aleksandr/A-6244-2014; Karyukhin, Andrey/J-3904-2014; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Olshevskiy, Alexander/I-1580-2016; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Mora Herrera, Maria Clemencia/L-3893-2016; Maneira, Jose/D-8486-2011; KHODINOV, ALEKSANDR/D-6269-2015; Goncalo, Ricardo/M-3153-2016; Gauzzi, Paolo/D-2615-2009; Gerbaudo, Davide/J-4536-2012; Tikhomirov, Vladimir/M-6194-2015; Chekulaev, Sergey/O-1145-2015; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; Carvalho, Joao/M-4060-2013; Mashinistov, Ruslan/M-8356-2015; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Wemans, Andre/A-6738-2012; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Mir, Lluisa-Maria/G-7212-2015; Riu, Imma/L-7385-2014; Cabrera Urban, Susana/H-1376-2015; Garcia, Jose /H-6339-2015; Della Pietra, Massimo/J-5008-2012; Cavalli-Sforza, Matteo/H-7102-2015; 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Prokoshin, Fedor/E-2795-2012; Dawson, Ian/K-6090-2013; Solfaroli Camillocci, Elena/J-1596-2012; Tudorache, Valentina/D-2743-2012; Marti-Garcia, Salvador/F-3085-2011; Castro, Nuno/D-5260-2011; Wolters, Helmut/M-4154-2013; Warburton, Andreas/N-8028-2013; De, Kaushik/N-1953-2013; Sukharev, Andrey/A-6470-2014; Lee, Jason/B-9701-2014 OI Osculati, Bianca Maria/0000-0002-7246-060X; Amorim, Antonio/0000-0003-0638-2321; Santos, Helena/0000-0003-1710-9291; Coccaro, Andrea/0000-0003-2368-4559; Vanyashin, Aleksandr/0000-0002-0367-5666; Ferrando, James/0000-0002-1007-7816; La Rosa, Alessandro/0000-0001-6291-2142; Moraes, Arthur/0000-0002-5157-5686; Smirnov, Sergei/0000-0002-6778-073X; Conde Muino, Patricia/0000-0002-9187-7478; Andreazza, Attilio/0000-0001-5161-5759; Boyko, Igor/0000-0002-3355-4662; Kuleshov, Sergey/0000-0002-3065-326X; Pina, Joao /0000-0001-8959-5044; Moorhead, Gareth/0000-0002-9299-9549; Orlov, Ilya/0000-0003-4073-0326; Petrucci, Fabrizio/0000-0002-5278-2206; Annovi, Alberto/0000-0002-4649-4398; Brooks, William/0000-0001-6161-3570; Stoicea, Gabriel/0000-0002-7511-4614; Doyle, Anthony/0000-0001-6322-6195; Smestad, Lillian/0000-0002-0244-8736; Giordani, Mario/0000-0002-0792-6039; Abdelalim, Ahmed Ali/0000-0002-2056-7894; Capua, Marcella/0000-0002-2443-6525; Di Micco, Biagio/0000-0002-4067-1592; Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; Doria, Alessandra/0000-0002-5381-2649; Veloso, Filipe/0000-0002-5956-4244; Gomes, Agostinho/0000-0002-5940-9893; Fassi, Farida/0000-0002-6423-7213; la rotonda, laura/0000-0002-6780-5829; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Monzani, Simone/0000-0002-0479-2207; Grancagnolo, Francesco/0000-0002-9367-3380; Korol, Aleksandr/0000-0001-8448-218X; Maio, Amelia/0000-0001-9099-0009; Fiolhais, Miguel/0000-0001-9035-0335; Karyukhin, Andrey/0000-0001-9087-4315; Anjos, Nuno/0000-0002-0018-0633; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Olshevskiy, Alexander/0000-0002-8902-1793; 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spagnolo, stefania/0000-0001-7482-6348; Camarri, Paolo/0000-0002-5732-5645; Tomasek, Lukas/0000-0002-5224-1936; Svatos, Michal/0000-0002-7199-3383; Peleganchuk, Sergey/0000-0003-0907-7592; Santamarina Rios, Cibran/0000-0002-9810-1816; Bosman, Martine/0000-0002-7290-643X; Ventura, Andrea/0000-0002-3368-3413; Livan, Michele/0000-0002-5877-0062; Mitsou, Vasiliki/0000-0002-1533-8886; Joergensen, Morten/0000-0002-6790-9361; Smirnova, Oxana/0000-0003-2517-531X; Fabbri, Laura/0000-0002-4002-8353; Villa, Mauro/0000-0002-9181-8048; Mikestikova, Marcela/0000-0003-1277-2596; Kuday, Sinan/0000-0002-0116-5494; Prokoshin, Fedor/0000-0001-6389-5399; Solfaroli Camillocci, Elena/0000-0002-5347-7764; Castro, Nuno/0000-0001-8491-4376; Wolters, Helmut/0000-0002-9588-1773; Warburton, Andreas/0000-0002-2298-7315; De, Kaushik/0000-0002-5647-4489; Lee, Jason/0000-0002-2153-1519 FU ANPCyT, At YerPhI, Armenia; ARC, Australia; BMWF, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union; ERC, European Union; NSRF, European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvII Foundation, Germany; GSRT, Greece; NSRF, Greece; ISF, Israel; MINERVA, Israel; GIF, Israel; DIP, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; GRICES, Portugal; FCT, Portugal; MERYS (MECTS), Romania; MES of Russia, Russian Federation; ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MVZT, Slovenia; DST/NRE, South Africa; MICINN, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America FX We acknowledge the support of ANPCyT, At YerPhI, Armenia; ARC, Australia; BMWF and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvII Foundation, Germany; GSRT and NSRF, Greece; ISF, MINERVA, GIF, DIP and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW, Poland; GRICES and FCT, Portugal; MERYS (MECTS), Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MVZT, Slovenia; DST/NRE, South Africa; MICINN, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. NR 36 TC 9 Z9 9 U1 6 U2 135 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JAN PY 2013 IS 1 AR 086 DI 10.1007/JHEP01(2013)086 PG 42 WC Physics, Particles & Fields SC Physics GA 098XY UT WOS:000315583600005 ER PT J AU Aad, G Abajyan, T Abbott, B Abdallah, J Khalek, SA Abdelalim, AA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Acharya, BS Adamczyk, L Adams, DL Addy, TN Adelman, J Adomeit, S Adragna, P Adye, T Aefsky, S Aguilar-Saavedra, JA Agustoni, M Aharrouche, M Ahlen, SP Ahles, F Ahmad, A Ahsan, M Aielli, G Akesson, TPA Akimoto, G Akimov, AV Alam, MS Alam, MA Albert, J Albrand, S Aleksa, M Aleksandrov, IN Alessandria, F Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Aliev, M Alimonti, G Alison, J Allbrooke, BMM Allport, PP Allwood-Spiers, SE Almond, J Aloisio, A Alon, R Alonso, A Alonso, F Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Amelung, C Ammosov, VV Dos Santos, SPA Amorim, A Amram, N Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Andrieux, ML Anduaga, XS Angelidakis, S Anger, P Angerami, A Anghinolfi, F Anisenkov, A Anjos, N Annovi, A Antonaki, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Aoun, S Bella, LA Apolle, R Arabidze, G Aracena, I Arai, Y Arce, ATH Arfaoui, S Arguin, JF Argyropoulos, S Arik, E Arik, M Armbruster, AJ Arnaez, O Arnal, V Arnault, C Artamonov, A Artoni, G Arutinov, D Asai, S Ask, S Asman, B Asquith, L Assamagan, K Astbury, A Atkinson, M Aubert, B Auge, E Augsten, K Aurousseau, M Avolio, G Avramidou, R Axen, D Azuelos, G Azuma, Y Baak, MA Baccaglioni, G Bacci, C Bach, AM Bachacou, H Bachas, K Backes, M Backhaus, M Mayes, JB Badescu, E Bagnaia, P Bahinipati, S Bai, Y Bailey, DC Bain, T Baines, JT Baker, OK Baker, MD Baker, S Balek, P Banas, E Banerjee, P Banerjee, S Banfi, D Bangert, A Bansal, V Bansil, HS Barak, L Baranov, SP Galtieri, AB Barber, T Barberio, EL Barberis, D Barbero, M Bardin, DY Barillari, T Barisonzi, M Barklow, T Barlow, N Barnett, BM Barnett, RM Baroncelli, A Barone, G Barr, AJ 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CA ATLAS Collaboration TI ATLAS search for new phenomena in dijet mass and angular distributions using pp collisions at root s=7 TeV SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering ID PARTON DISTRIBUTIONS; HADRON COLLIDERS; STANDARD MODEL; JET PRODUCTION; CHIRAL COLOR; 1 FB(-1); DETECTOR; PHYSICS; NEUTRINO; LEPTON AB Mass and angular distributions of dijets produced in LHC proton-proton collisions at a centre-of-mass energy root s = 7TeV have been studied with the ATLAS detector using the full 2011 data set with an integrated luminosity of 4.8 fb(-1). Dijet masses up to similar to 4.0TeV have been probed. No resonance-like features have been observed in the dijet mass spectrum, and all angular distributions are consistent with the predictions of QCD. Exclusion limits on six hypotheses of new phenomena have been set at 95% CL in terms of mass or energy scale, as appropriate. 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M.; Kaneda, M.; Kaplon, J.; Kerschen, N.; Klioutchnikova, T.; Koeneke, K.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malaescu, B.; Malyukov, S.; Mapelli, A.; Mapelli, L.; Marshall, Z.; Martin, B.; Messina, A.; Michal, S.; Molfetas, A.; Morley, A. K.; Mornacchi, G.; Muenstermann, D.; Nairz, A. M.; Nakahama, Y.; Negri, G.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Ohm, C. C.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Petersen, J.; Piacquadio, G.; Pommes, K.; Poppleton, A.; Bueso, X. Portell; Poulard, G.; Prasad, S.; Raymond, M.; Rembser, C.; Dos Santos, D. Roda; Roe, S.; Salek, D.; Salzburger, A.; Savu, D. O.; Schlenker, S.; Schott, M.; Sfyrla, A.; Spigo, G.; Spiwoks, R.; Stewart, G. A.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van der Ster, D.; van Eldik, N.; Vandelli, W.; Veness, R.; Vinek, E.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. 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[Han, L.; Jiang, Y.; Li, B.; Li, S.; Liu, M.; Liu, Y.; Peng, H.; Wu, Y.; Xu, C.; Xu, L.; Zhang, D.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Feng, C.; Ge, P.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Toro, R. Camacho; Cinca, D.; Donini, J.; Febbraro, R.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Vazeille, F.] Clermont Univ, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Toro, R. Camacho; Cinca, D.; Donini, J.; Febbraro, R.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Toro, R. Camacho; Cinca, D.; Donini, J.; Febbraro, R.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Vazeille, F.] Univ Clermont Ferrand, Photochim Mol & Macromol Lab, CNRS, IN2P3, F-63177 Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Brooijmans, G.; Chen, Y.; Dodd, J.; Grau, N.; Guo, J.; Hu, D.; Hughes, E. W.; Nikiforou, N.; Parsons, J. A.; Penson, A.; Perez, K.; Reale, V. Perez; Scherzer, M. I.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Williams, E.; Willis, W.; Wulf, E.; Zivkovic, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Boelaert, N.; Dam, M.; Gregersen, K.; Hansen, J. R.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Heisterkamp, S.; Jakobsen, S.; Loevschall-Jensen, A. E.; Jez, P.; Joergensen, M. D.; Kadlecik, P.; Klinkby, E. B.; Lundquist, J.; Mackeprang, R.; Mehlhase, S.; Petersen, T. C.; Simonyan, M.; Thomsen, L. A.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; Fazio, S.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Morello, G.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, INFN Grp Coll Cosenza, Arcavacata Di Rende, Italy. [Capua, M.; Crosetti, G.; Fazio, S.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Morello, G.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Banas, E.; Blocki, J.; de Renstrom, P. A. Bruckman; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Malecki, P.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Turala, M.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.; Zemla, A.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Yagci, K. Dindar; Firan, A.; Hoffman, J.; Joffe, D.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Rios, R. R.; Sekula, S. J.; Stroynowski, R.; Wang, H.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Ahsan, M.; Izen, J. M.; Lou, X.; Reeves, K.; Wong, W. C.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Kuutmann, E. Bergeaas; Bloch, I.; Dassoulas, J. A.; Dietrich, J.; Ehrenfeld, W.; Ferrara, V.; Fischer, G.; Friedrich, C.; Glazov, A.; Goebel, M.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K-J.; Gregor, I. M.; Hiller, K. H.; Huettmann, A.; Belenguer, M. Jimenez; Johnert, S.; Karnevskiy, M.; Katzy, J.; Kono, T.; Kuhl, T.; Lange, C.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Cavalcanti, T. Perez; Petschull, D.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Zhu, H.] DESY, Hamburg, Germany. [Argyropoulos, S.; Kuutmann, E. Bergeaas; Bloch, I.; Dassoulas, J. A.; Dietrich, J.; Ehrenfeld, W.; Ferrara, V.; Fischer, G.; Friedrich, C.; Glazov, A.; Goebel, M.; Fajardo, L. S. Gomez; Da Costa, J. Goncalves Pinto Firmino; Grahn, K-J.; Gregor, I. M.; Hiller, K. H.; Huettmann, A.; Belenguer, M. Jimenez; Johnert, S.; Karnevskiy, M.; Katzy, J.; Kono, T.; Kuhl, T.; Lange, C.; Lobodzinska, E.; Ludwig, D.; Maettig, S.; Medinnis, M.; Moenig, K.; Naumann, T.; Cavalcanti, T. Perez; Petschull, D.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Zhu, H.] DESY, Zeuthen, Germany. [Bunse, M.; Esch, H.; Goessling, C.; Hirsch, F.; Jung, C. A.; Klingenberg, R.; Reisinger, I.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Czodrowski, P.; Friedrich, F.; Goepfert, T.; Kobel, M.; Leonhardt, K.; Ludwig, A.; Mader, W. F.; Morgenstern, M.; Prudent, X.; Rudolph, C.; Schnoor, U.; Schwierz, R.; Seifert, F.; Steinbach, P.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Ebenstein, W. L.; Fowler, A. J.; Ko, B. R.; Kotwal, A.; Kruse, M. K.; Oh, S. H.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Buckley, A. G.; Clark, P. J.; Debenedetti, C.; Harrington, R. D.; Martin, V. J.; O'Brien, B. J.; Schaelicke, A.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Cerutti, F.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.; Volpi, G.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Aad, G.; Ahles, F.; Barber, T.; Bernhard, R.; Boehler, M.; Bruneliere, R.; Christov, A.; Consorti, V.; Fehling-Kaschek, M.; Flechl, M.; Hartert, J.; Herten, G.; Horner, S.; Jakobs, K.; Janus, M.; Kononov, A. I.; Kuehn, S.; Lai, S.; Landgraf, U.; Lohwasser, K.; Ludwig, I.; Ludwig, J.; Mahboubi, K.; Mohr, W.; Nilsen, H.; Parzefall, U.; Rammensee, M.; Rave, T. C.; Rurikova, Z.; Schmidt, E.; Schumacher, M.; Siegert, F.; Stoerig, K.; Sundermann, J. E.; Temming, K. K.; Thoma, S.; Tsiskaridze, V.; Venturi, M.; Vivarelli, I.; von Radziewski, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Winkelmann, S.; Xie, S.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Abdelalim, A. A.; Alexandre, G.; Backes, M.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; Blondel, A.; Bucci, F.; Clark, A.; Dao, V.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Iacobucci, G.; La Rosa, A.; Lister, A.; Latour, B. Martin Dit; Mermod, P.; Herrera, C. Mora; Nektarijevic, S.; Nikolics, K.; Pasztor, G.; Picazio, A.; Pohl, M.; Rosbach, K.; Rosselet, L.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Caso, C.; Dameri, M.; Darbo, G.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Univ Genoa, INFN Sez Genova, Genoa, Italy. [Barberis, D.; Caso, C.; Dameri, M.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Chikovani, L.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Khubua, J.; Mchedlidze, G.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Bussey, P.; Buttar, C. M.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Edwards, N. C.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Kar, D.; Kenyon, M.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Robson, A.; Saxon, D. H.; Smith, K. M.; St Denis, R. D.; Steele, G.; Thompson, A. S.; Wraight, K.; Wright, M.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bierwagen, K.; Blumenschein, U.; Brandt, O.; Erdmann, J.; Evangelakou, D.; George, M.; Grosse-Knetter, J.; Guindon, S.; Hamer, M.; Hensel, C.; Keil, M.; Knue, A.; Kohn, F.; Krieger, N.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Mann, A.; Meyer, J.; Morel, J.; Nackenhorst, O.; Pashapour, S.; Quadt, A.; Roe, A.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Uhrmacher, M.; Schroeder, T. Vazquez; Weingarten, J.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Andrieux, M-L.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Stark, J.; Sun, X.; Trocme, B.; Wang, J.; Weydert, C.] Univ Grenoble 1, Lab Phys Subatom & Cosmol, Grenoble, France. [Albrand, S.; Andrieux, M-L.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Stark, J.; Sun, X.; Trocme, B.; Wang, J.; Weydert, C.] CNRS, IN2P3, Grenoble, France. [Albrand, S.; Andrieux, M-L.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Stark, J.; Sun, X.; Trocme, B.; Wang, J.; Weydert, C.] Inst Natl Polytech Grenoble, F-38031 Grenoble, France. [Addy, T. N.; Harvey, A.; McFarlane, K. W.; Shin, T.; Vassilakopoulos, V. I.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Belloni, A.; Catastini, P.; Conti, G.; Franklin, M.; Huth, J.; Jeanty, L.; Kagan, M.; Mateos, D. Lopez; Outschoorn, V. Martinez; Mercurio, K. M.; Mills, C.; Morii, M.; Skottowe, H. P.; Smith, B. C.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Anders, G.; Andrei, V.; Davygora, Y.; Dietzsch, T. A.; Dunford, M.; Geweniger, C.; Hanke, P.; Henke, M.; Khomich, A.; Kluge, E. -E.; Lang, V. S.; Lendermann, V.; Lepold, F.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Kugel, A.; Maenner, R.; Schroer, N.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Cwetanski, P.; Evans, H.; Gagnon, P.; Jain, V.; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Price, D.; Whittington, D.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Epp, B.; Jussel, P.; Kneringer, E.; Kuhn, D.; Lukas, W.; Rudolph, G.] Leopold Eranzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Behera, P. K.; Limper, M.; Mallik, U.; Pylypchenko, Y.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Rosenberg, E. I.; Ruiz-Martinez, A.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Aleksandrov, I. N.; Anisenkov, A.; Bardin, D. Y.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Grigalashvili, N.; Huseynov, N.; Kalinovskaya, L. V.; Kazarinov, M. Y.; Kekelidze, G. D.; Kharchenko, D.; Khramov, E.; Kolesnikov, V.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Pozdnyakov, V.; Rumyantsev, L.; Rusakovich, N. A.; Sadykov, R.; Shiyakova, M.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.; Zimin, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Arai, Y.; Doi, Y.; Haruyama, T.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Makida, Y.; Manabe, A.; Mitsui, S.; Nagano, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Hayakawa, T.; King, M.; Kishimoto, T.; Kitamura, T.; Kurashige, H.; Matsushita, T.; Ochi, A.; Suzuki, Y.; Takeda, H.; Tani, K.; Watanabe, I.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Sasao, N.; Sumida, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Davidson, R.; de Mora, L.; Dearnaley, W. J.; Fox, H.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Bianco, M.; Cataldi, G.; Chiodini, G.; Gorini, E.; Grancagnolo, F.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Univ Salento, INFN Sez Lecce, Lecce, Italy. [Bianco, M.; Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; Cowan, G.; D'Onofrio, M.; Dervan, P.; Greenshaw, T.; Gwilliam, C. B.; Hayward, H. S.; Jackson, J. N.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kluge, T.; Kretzschmar, J.; Laycock, P.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Sellers, G.; Vossebeld, J. H.; Waller, P.; Wrona, B.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Dolenc, I.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Dolenc, I.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia. [Adragna, P.; Bona, M.; Carter, A. A.; Cerrito, L.; Eisenhandler, E.; Ellis, K.; Goddard, J. R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Poll, J.; Rizvi, E.; Salamanna, G.; Castanheira, M. Teixeira Dias; Wiglesworth, C.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Alam, M. A.; Berry, T.; Boisvert, V.; Brooks, T.; Cantrill, R.; Duguid, L.; Edwards, C. A.; George, S.; Goncalo, R.; Hayden, D.; Vazquez, J. G. Panduro; Pastore, Fr.; Rose, M.; Spano, F.; Strong, J. A.; Teixeira-Dias, P.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Baker, S.; Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Chislett, R. T.; Christidi, I. A.; Cooper, B. D.; Davison, A. R.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Lambourne, L.; Monk, J.; Nash, M.; Nurse, E.; Prabhu, R.; Sherwood, P.; Simmons, B.; Taylor, C.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Cavalleri, P.; Chareyre, E.; Davignon, O.; De Cecco, S.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph.; Theveneaux-Pelzer, T.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Cavalleri, P.; Chareyre, E.; Davignon, O.; De Cecco, S.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph.; Theveneaux-Pelzer, T.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Cavalleri, P.; Chareyre, E.; Davignon, O.; De Cecco, S.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph.; Theveneaux-Pelzer, T.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] CNRS, IN2P3, Paris, France. [Ahmad, A.; Akesson, T. P. A.; Alonso, A.; Bocchetta, S. S.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Jarlskog, G.; Lundberg, B.; Lytken, E.; Meirose, B.; Mjoernmark, J. U.; Smirnova, O.] Lund Univ, Fysiska Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Labarga, L.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Aharrouche, M.; Arnaez, O.; Blum, W.; Buscher, V.; Caputo, R.; Eckweiler, S.; Edmonds, K.; Ellinghaus, F.; Ertel, E.; Fiedler, F.; Fleckner, J.; Goeringer, C.; Handel, C.; Hohlfeld, M.; Hsu, P. J.; Ji, W.; Kawamura, G.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lungwitz, M.; Masetti, L.; Meyer, C.; Moreno, D.; Mueller, T.; Neusiedl, A.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schroeder, C.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Almond, J.; Borri, M.; Brown, G.; Chavda, V.; Cox, B. E.; Da Via, C.; Duerdoth, I. P.; Forti, A.; Howarth, J.; Ibbotson, M.; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Marx, M.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Pilkington, A. D.; Robinson, J. E. M.; Schwanenberger, C.; Snow, S. W.; Watts, S.; Woudstra, M. J.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aoun, S.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Odier, J.; Pralavorio, P.; Rozanov, A.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aoun, S.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Odier, J.; Pralavorio, P.; Rozanov, A.; Talby, M.; Tannoury, N.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Brau, B.; Colon, G.; Dallapiccola, C.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Caron, B.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Dobbs, M.; Dufour, M-A.; Klemetti, M.; Mc Donald, J.; Robertson, S. H.; Rios, C. Santamarina; Schram, M.; Stockton, M. C.; Vachon, B.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Davidson, N.; Diglio, S.; Hamano, K.; Jennens, D.; Kubota, T.; Limosani, A.; Moorhead, G. F.; Hanninger, G. Nunes; Phan, A.; Shao, Q. T.; Tan, K. G.; Taylor, G. N.; Thong, W. M.; Volpi, M.; White, M. J.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Armbruster, A. J.; Borroni, S.; Chapman, J. W.; Cirilli, M.; Dai, T.; Diehl, E. B.; Ferretti, C.; Goldfarb, S.; Harper, D.; Levin, D.; Li, X.; Liu, H.; Liu, J. B.; Liu, L.; Mc Kee, S. P.; Neal, H. A.; Panikashvili, N.; Purdham, J.; Qian, J.; Scheirich, D.; Thun, R. P.; Walch, S.; Wilson, A.; Wooden, G.; Wu, Y.; Yang, H.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Fedorko, W.; Hauser, R.; Holzbauer, J. L.; Huston, J.; Linnemann, J. T.; Martin, B.; Miller, R. J.; Pope, B. G.; Schwienhorst, R.; Stelzer, H. 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[Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Banerjee, P.; Bouchami, J.; Davies, M.; Giunta, M.; Leroy, C.; Martin, J. P.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.] Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys ITEP, Moscow, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.] Moscow Engn & Phys Inst MEPhI, Moscow, Russia. [Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Beale, S.; Becker, S.; Biebel, O.; Bortfeldt, J.; Calfayan, P.; de Graat, J.; Duckeck, G.; Ebke, J.; Elmsheuser, J.; Engl, A.; Galea, C.; Heller, C.; Hertenberger, R.; Kummer, C.; Legger, F.; Lichtnecker, M.; Lorenz, J.; Mameghani, R.; Mueller, T. A.; Nunnemann, T.; Oakes, L. B.; Rauscher, F.; Reznicek, P.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Schieck, J.; Serfon, C.; Staude, A.; Vladoiu, D.; Walker, R.; Will, J. Z.; Zhuang, X.; Zibell, A.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Beimforde, M.; Bethke, S.; Bittner, B.; Bronner, J.; Capriotti, D.; Compostella, G.; Cortiana, G.; Dubbert, J.; Flowerdew, M. J.; Giovannini, P.; Ince, T.; Jantsch, A.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kotov, S.; Kroha, H.; Macchiolo, A.; Manfredini, A.; Menke, S.; Moser, H. G.; Nagel, M.; Nisius, R.; Oberlack, H.; Pahl, C.; Pospelov, G. E.; Potrap, I. N.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Stern, S.; Stonjek, S.; Vanadia, M.; von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.; Zhuravlov, V.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Shimizu, S.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Capasso, L.; Carlino, G.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; della Volpe, D.; Di Donato, C.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Patricelli, S.; Sanchez, A.; Sekhniaidze, G.] Univ Naples Federico II, INFN Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Capasso, L.; Chiefari, G.; della Volpe, D.; Di Donato, C.; Giordano, R.; Merola, L.; Patricelli, S.; Sanchez, A.] Univ Naples Federico II, Dipartimento Sci Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Chelstowska, M. A.; De Groot, N.; Filthaut, F.; Klok, P. F.; Koenig, A. C.; Koetsveld, F.; Salvucci, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Doxiadis, A. D.; Ferrari, P.; Garitaonandia, H.; Geerts, D. A. A.; Gosselink, M.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kayl, M. S.; Klous, S.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Luijckx, G.; Mahlstedt, J.; Massaro, G.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Pani, P.; Rijpstra, M.; Ruckstuhl, N.; Ta, D.; Tsiakiris, M.; Turlay, E.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van der Poel, E.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.] Nikhef Natl Inst Subatom Phys, Amsterdam, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Doxiadis, A. D.; Ferrari, P.; Garitaonandia, H.; Geerts, D. A. A.; Gosselink, M.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kayl, M. S.; Klous, S.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Luijckx, G.; Mahlstedt, J.; Massaro, G.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Pani, P.; Rijpstra, M.; Ruckstuhl, N.; Ta, D.; Tsiakiris, M.; Turlay, E.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van der Poel, E.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.] Univ Amsterdam, Amsterdam, Netherlands. [Calkins, R.; Chakraborty, D.; Cole, S.; de Lima, J. G. Rocha; Suhr, C.; Yurkewicz, A.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL USA. [Anisenkov, A.; Beloborodova, O.; Bobrovnikov, V. B.; Bogdanchikov, A.; Kazanin, V. A.; Kolachev, G. M.; Korol, A.; Malyshev, V.; Maslennikov, A. L.; Maximov, D. A.; Orlov, I.; Peleganchuk, S. V.; Schamov, A. G.; Skovpen, K.; Soukharev, A.; Talyshev, A.; Tikhonov, Y. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Budick, B.; Casadei, D.; Cranmer, K.; Haas, A.; van Huysduynen, L. Hooft; Kaplan, B.; Konoplich, R.; Krasznahorkay, A.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.; Prokofiev, K.; Zhao, L.] NYU, Dept Phys, New York, NY 10003 USA. [Fisher, M. J.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Raas, M.; Rahimi, A. M.; Strang, M.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Gutierrez, P.; Jana, D. K.; Marzin, A.; Meera-Lebbai, R.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Snow, J.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Khanov, A.; Rizatdinova, F.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Hamal, P.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Bruncko, D.; Potter, C. T.; Ptacek, E.; Radloff, P.; Reinsch, A.; Searcy, J.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Andari, N.; Arnault, C.; Auge, E.; Barrillon, P.; Benoit, M.; Binet, S.; Bourdarios, C.; De La Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Loscutoff, P.; Lounis, A.; Makovec, N.; Matricon, P.; Niedercorn, F.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Ruan, X.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Teinturier, M.; Veillet, J. J.; Wicek, F.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Andari, N.; Arnault, C.; Auge, E.; Barrillon, P.; Benoit, M.; Binet, S.; Bourdarios, C.; De La Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Loscutoff, P.; Lounis, A.; Makovec, N.; Matricon, P.; Niedercorn, F.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Ruan, X.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Teinturier, M.; Veillet, J. J.; Wicek, F.; Zerwas, D.; Zhang, Z.] CNRS, IN2P3, F-91405 Orsay, France. [Hanagaki, K.; Hirose, M.; Lee, J. S. H.; Meguro, T.; Nomachi, M.; Okamura, W.; Sugaya, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Buran, T.; Cameron, D.; Gjelsten, B. K.; Gramstad, E.; Lund, E.; Ould-Saada, F.; Pajchel, K.; Read, A. L.; Rohne, O.; Samset, B. H.; Smestad, L.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Apolle, R.; Barr, A. J.; Boddy, C. R.; Brandt, G.; Buchanan, J.; Buckingham, R. M.; Cooper-Sarkar, A. M.; Dafinca, A.; Davies, E.; Gallas, E. J.; Gwenlan, C.; Hall, D.; Hays, C. P.; Howard, J.; Huffman, T. B.; Issever, C.; King, R. S. B.; Kogan, L. A.; Korn, A.; Larner, A.; Lewis, A.; Liang, Z.; Livermore, S. S. A.; Mattravers, C.; Nickerson, R. B.; Pinder, A.; Robichaud-Veronneau, A.; Ryder, N. C.; Short, D.; Tseng, J. C-L.; Vickey, T.; Viehhauser, G. H. A.; Weidberg, A. R.; Whitehead, S. R.; Young, C. J.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Colombo, T.; Conta, C.; Ferrari, R.; Franchino, S.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Uslenghi, M.; Vercesi, V.] Univ Pavia, INFN Sez Pavia, I-27100 Pavia, Italy. [Colombo, T.; Conta, C.; Ferrari, R.; Franchino, S.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Uslenghi, M.; Vercesi, V.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Alison, J.; Brendlinger, K.; Degenhardt, J.; Dressnandt, N.; Fratina, S.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Keener, P. T.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Newcomer, F. M.; Olivito, D.; Ospanov, R.; Reece, R.; Saxon, J.; Schaefer, D.; Stahlman, J.; Thomson, E.; Van Berg, R.; Wagner, P.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Bertolucci, F.; Cascella, M.; Cavasinni, V.; Crescioli, F.; Del Prete, T.; Dotti, A.; Roda, C.; Sarri, F.; White, S.; Zinonos, Z.] Univ Pisa, INFN Sez Pisa, Pisa, Italy. [Bertolucci, F.; Cascella, M.; Cavasinni, V.; Crescioli, F.; Del Prete, T.; Dotti, A.; Roda, C.; Sarri, F.; White, S.; Zinonos, Z.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Boudreau, J.; Cleland, W.; Escobar, C.; Kittelmann, T.; Mueller, J.; Prieur, D.; Savinov, V.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Anjos, N.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Sargedas De Sousa, M. J. Da Cunha; Do Valle Wemans, A.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Jorge, P. M.; Lopes, L.; Machado Miguens, J.; Maio, A.; Maneira, J.; Oliveira, M.; Onofre, A.; Palma, A.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Veloso, F.; Wolters, H.] LIP, Lab Instrumentacao & Fis Expt Particulas, P-1000 Lisbon, Portugal. [Amor Dos Santos, S. P.; Amorim, A.; Anjos, N.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Sargedas De Sousa, M. J. Da Cunha; Do Valle Wemans, A.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Jorge, P. M.; Lopes, L.; Machado Miguens, J.; Maio, A.; Maneira, J.; Oliveira, M.; Onofre, A.; Palma, A.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Veloso, F.; Wolters, H.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. [Bohm, J.; Chudoba, J.; Gallus, P.; Gunther, J.; Jakoubek, T.; Juranek, V.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Marcisovsky, M.; Mikestikova, M.; Myska, M.; Nemecek, S.; Ruzicka, P.; Schovancova, J.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Tic, T.; Valenta, J.; Vrba, V.; Zeman, M.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Balek, P.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Kodys, P.; Leitner, R.; Novakova, J.; Rybar, M.; Spousta, M.; Strachota, P.; Suk, M.; Sykora, T.; Tas, P.; Valkar, S.; Vorobel, V.; Wilhelm, I.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Augsten, K.; Holy, T.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Kral, V.; Krejci, F.; Pospisil, S.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solar, M.; Solc, J.; Sopko, V.; Sopko, B.; Stekl, I.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Ammosov, V. V.; Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Ivashin, A. V.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.; Zmouchko, V. V.] State Res Ctr Inst High Energy Phys, Protvino, Russia. [Adye, T.; Apolle, R.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Gillman, A. R.; Haywood, S. J.; Kirk, J.; Mattravers, C.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Nash, M.; Norton, P. R.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Benslama, K.; Smit, G. V. Ybeles] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Artoni, G.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Pedis, D.; De Salvo, A.; De Zorzi, G.; Falciano, S.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Rossi, E.; Tehrani, F. Safai; Sidoti, A.; Camillocci, E. Solfaroli; Vari, R.; Veneziano, S.; Zanello, L.] Univ Roma La Sapienza, INFN Sez Roma 1, Rome, Italy. [Artoni, G.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; De Zorzi, G.; Dionisi, C.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Rossi, E.; Camillocci, E. Solfaroli; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Di Simone, A.; Liberti, B.; Marchese, F.; Mazzaferro, L.; Salamon, A.; Santonico, R.] Univ Roma Tor Vergata, INFN Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Cattani, G.; Di Ciaccio, A.; Di Simone, A.; Marchese, F.; Mazzaferro, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Branchini, P.; Ceradini, F.; Di Luise, S.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Stanescu, C.] Univ Roma Tre, INFN Sez Roma Tre, Rome, Italy. [Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Luise, S.; Orestano, D.; Pastore, F.; Petrucci, F.] Univ Roma Tre, Dipartimento Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.; Lablak, S.] Univ Hassan 2, Fac Sci Ain Chock, Reseau Univ Phys Hautes Energies, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA Marrakech, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Abreu, H.; Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Bolnet, N. M.; Boonekamp, M.; Chevalier, L.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Gauthier, L.; Giraud, P. F.; Guyot, C.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Legendre, M.; Maiani, C.; Mal, P.; Ramos, J. A. Manjarres; Mansoulie, B.; Meyer, J-P.; Mijovic, L.; Morange, N.; Mountricha, E.; Hong, V. Nguyen Thi; Nicolaidou, R.; Ouraou, A.; Resende, B.; Royon, C. R.; Schoeffel, L.; Schune, Ph.; Schwindling, J.; Simard, O.; Virchaux, M.; Vranjes, N.; Xiao, M.; Xu, C.] CEA Saclay, DSM, IRFU, F-91191 Gif Sur Yvette, France. [Chouridou, S.; Damiani, D. S.; Grillo, A. A.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Mitrevski, J.; Nielsen, J.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Beckingham, M.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Keller, J. S.; Lubatti, H. J.; Rompotis, N.; Rothberg, J.; Verducci, M.; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Duxfield, R.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Mayne, A.; Mcfayden, J. A.; Miyagawa, P. S.; Owen, S.; Paganis, E.; Suruliz, K.; Tovey, D. R.; Tsionou, D.; Tua, A.; Xu, D.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Holder, M.; Ibragimov, I.; Rammes, M.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Dawe, E.; Godfrey, J.; Kvita, J.; O'Neil, D. C.; Petteni, M.; Stelzer, B.; Trottier-McDonald, M.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Mayes, J. Backus; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Butler, B.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Grenier, P.; Hansson, P.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nelson, T. K.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Smith, D.; Strauss, E.; Su, D.; Tanasijczuk, A. J.; Wilson, M. G.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Batkova, L.; Blazek, T.; Federic, P.; Pecsy, M.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Ferencei, J.; Kladiva, E.; Seman, M.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Aurousseau, M.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Carrillo-Montoya, G. D.; Hamilton, A.; Leney, K. J. C.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Asman, B.; Bendtz, K.; Bohm, C.; Clement, C.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Holmgren, S. O.; Johansen, M.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Papadelis, A.; Sellden, B.; Silverstein, S. B.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Asman, B.; Bendtz, K.; Clement, C.; Gellerstedt, K.; Hellman, S.; Johansen, M.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Ahmad, A.; Arfaoui, S.; Devetak, E.; DeWilde, B.; Engelmann, R.; Farley, J.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Li, H.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Ahmad, A.; Arfaoui, S.; Devetak, E.; DeWilde, B.; Engelmann, R.; Farley, J.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Li, H.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Bartsch, V.; De Santo, A.; Martin-Haugh, S.; Potter, C. J.; Rose, A.; Salvatore, F.; Santoyo Castillo, I.; Sutton, M. R.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Bangert, A.; Cuthbert, C.; Patel, N.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Waugh, A. T.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Chu, M. L.; Hou, S.; Jamin, D. O.; Lee, S. C.; Lin, S. C.; Liu, D.; Mazini, R.; Meng, Z.; Ren, Z. L.; Soh, D. A.; Teng, P. K.; Wang, J.; Wang, S. M.; Weng, Z.; Zhang, D.; Zhou, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Harpaz, S. Behar; Kajomovitz, E.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; Vallecorsa, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Bella, G.; Benary, O.; Benhammou, Y.; Etzion, E.; Gershon, A.; Ginzburg, J.; Guttman, N.; Hod, N.; Munwes, Y.; Oren, Y.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Iliadis, D.; Kordas, K.; Kouskoura, V.; Nomidis, I.; Petridis, A.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, K.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yamazaki, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, K.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yamazaki, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Ishitsuka, M.; Jinnouchi, O.; Kanno, T.; Kuze, M.; Nagai, R.; Nobe, T.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Bailey, D. C.; Bain, T.; Brelier, B.; Cheung, S. L.; Dhaliwal, S.; Farooque, T.; Fatholahzadeh, B.; Gibson, A.; Guo, B.; Ilic, N.; Keung, J.; Krieger, P.; Orr, R. S.; Rezvani, R.; Rosenbaum, G. A.; Savard, P.; Sinervo, P.; Spreitzer, T.; Tardif, D.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Fortin, D.; Gingrich, D. M.; Koutsman, A.; Losty, M. J.; Nugent, I. M.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hanawa, K.; Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Kurata, M.; Nagai, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Napier, A.; Rolli, S.; Sliwa, K.; Todorova-Nova, S.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Loureiro, K. F.; Mendoza Navas, L.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Farrell, S.; Eschrich, I. Gough; Lankford, A. J.; Magnoni, L.; Mete, A. S.; Nelson, A.; Scannicchio, D. A.; Schernau, M.; Taffard, A.; Toggerson, B.; Unel, G.; Werth, M.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Pinamonti, M.; Shaw, K.; Soualah, R.] INFN Grp Collegato Udine, Udine, Italy. [Acharya, B. S.; Pinamonti, M.] ICIP, Trieste, Italy. [Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Giordani, M. P.; Shaw, K.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Coggeshall, J.; Cortes-Gonzalez, A.; Errede, D.; Errede, S.; Lie, K.; Liss, T. M.; McCarn, A.; Neubauer, M. S.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Brenner, R.; Buszello, C. P.; Coniavitis, E.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Pelikan, D.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Anisenkov, A.; Annovi, A.; Antonov, A.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Microelect Barcelona, IMB CNM, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; March, L.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] CSIC, Valencia, Spain. [Anisenkov, A.; Axen, D.; Gay, C.; Gecse, Z.; Loh, C. W.; Mills, W. J.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Astbury, A.; Bansal, V.; Berghaus, F.; Courneyea, L.; Fincke-Keeler, M.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Lessard, J-R.; Marino, C. P.; Martyniuk, A. C.; McPherson, R. A.; Ouellette, E. A.; Plamondon, M.; Sobie, R.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Farrington, S. M.; Jones, G.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Kimura, N.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Alon, R.; Barak, L.; Bressler, S.; Citron, Z. H.; Duchovni, E.; Frank, T.; Gross, E.; Groth-Jensen, J.; Klier, A.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Milstein, D.; Roth, I.; Silbert, O.; Smakhtin, V.; Vitells, O.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Hernandez, A. M. Castaneda; Castaneda-Miranda, E.; Chen, X.; Di Mattia, A.; Dos Anjos, A.; Fang, Y.; Castillo, L. R. Flores; Gabizon, O.; Gutzwiller, O.; Ji, H.; Ju, X.; Kashif, L.; Ma, L. L.; Garcia, B. R. Mellado; Ming, Y.; Pan, Y. B.; Morales, M. I. Pedraza; Sarangi, T.; Wang, H.; Wiedenmann, W.; Wu, S. L.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Fleischmann, P.; Meyer, J.; Redelbach, A.; Siragusa, G.; Stroehmer, R.; Trefzger, T.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Barisonzi, M.; Becker, A. K.; Becks, K. H.; Boek, J.; Braun, H. M.; Cornelissen, T.; Duda, D.; Fleischmann, S.; Flick, T.; Gerlach, P.; Glitza, K. W.; Gorfine, G.; Hamacher, K.; Harenberg, T.; Henss, T.; Hirschbuehl, D.; Kalinin, S.; Kersten, S.; Khoroshilov, A.; Kohlmann, S.; Lantzsch, K.; Lenzen, G.; Maettig, P.; Mechtel, M.; Neumann, M.; Pataraia, S.; Sandhoff, M.; Sartisohn, G.; Schultes, J.; Sturm, P.; Voss, T. T.; Wagner, W.; Wahlen, H.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany. [Adelman, J.; Baker, O. K.; Bedikian, S.; Almenar, C. Cuenca; Cummings, J.; Czyczula, Z.; Demers, S.; Garberson, F.; Golling, T.; Guest, D.; Henrichs, A.; Lagouri, T.; Lee, L.; Loginov, A.; Sherman, D.; Tipton, P.; Wall, R.; Walsh, B.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Biscarat, C.; Cogneras, E.; Quinonez, F.; Rahal, G.] Ctr Calcul, Inst Natl Phys Nucl & Phys Particules IN2P3, Villeurbanne, France. [Maio, A.; Pina, J.] Univ Lisbon, Fac Ciencias, P-1699 Lisbon, Portugal. [Maio, A.; Pina, J.] Univ Lisbon, CFNUL, P-1699 Lisbon, Portugal. [Bawa, H. S.; Gao, Y. S.; Lowe, A. J.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beloborodova, O.; Maximov, D. A.; Talyshev, A.; Tikhonov, Y. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Carvalho, J.; Fiolhais, M. C. N.; Oliveira, M.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Hernandez, A. M. Castaneda] UASLP, Dept Phys, San Luis Potosi, Mexico. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Corriveau, F.; McPherson, R. A.; Robertson, S. H.; Sobie, R.; Teuscher, R. J.] Inst Particle Phys IPP, Toronto, ON, Canada. [Demirkoz, B.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Dhullipudi, R.; Greenwood, Z. D.; Sawyer, L.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Do Valle Wemans, A.] Univ Nova Lisboa, Dep Fis, Caparica, Portugal. [Do Valle Wemans, A.] Univ Nova Lisboa, Fac Clencias & Tecnol, CEFTTEC, Caparica, Portugal. [Dobson, E.] UCL, Dept Phys & Astron, London, England. [Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Huseynov, N.] Azerbaijan Acad Sci, Inst Phys, Baku 370143, Azerbaijan. [Kono, T.; Wildt, M. A.] Univ Hamburg, Inst Expt Phys, Hamburg, Germany. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Carvalho, J.; Fiolhais, M. C. N.; Oliveira, M.; Wolters, H.] Aix Marseille Univ, CPPM, Marseille, France. [Carvalho, J.; Fiolhais, M. C. N.; Oliveira, M.; Wolters, H.] CNRS, IN2P3, Marseille, France. [Liang, Z.; Weng, Z.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou, Peoples R China. [Lin, S. C.] Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Meng, Z.] Shandong Univ, Sch Phys, Jinan City, Shandong, Peoples R China. [Messina, A.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Nessi, M.; Soh, D. A.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Park, W.; Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Pasztor, G.; Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Perez, K.] CALTECH, Pasadena, CA 91125 USA. [Richter-Was, E.] Jagiellonian Univ, Inst Phys, Krakow, Poland. [Spousta, M.] Columbia Univ, Nevis Lab, Irvington, NY USA. RP Aad, G (reprint author), Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. RI Yang, Haijun/O-1055-2015; Monzani, Simone/D-6328-2017; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Olshevskiy, Alexander/I-1580-2016; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Mora Herrera, Maria Clemencia/L-3893-2016; Maneira, Jose/D-8486-2011; KHODINOV, ALEKSANDR/D-6269-2015; Gauzzi, Paolo/D-2615-2009; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Kartvelishvili, Vakhtang/K-2312-2013; Prokoshin, Fedor/E-2795-2012; Dawson, Ian/K-6090-2013; Solfaroli Camillocci, Elena/J-1596-2012; Tudorache, Valentina/D-2743-2012; Marti-Garcia, Salvador/F-3085-2011; Wolters, Helmut/M-4154-2013; Warburton, Andreas/N-8028-2013; De, Kaushik/N-1953-2013; Sukharev, Andrey/A-6470-2014; Lee, Jason/B-9701-2014; Robson, Aidan/G-1087-2011; Chekulaev, Sergey/O-1145-2015; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; Carvalho, Joao/M-4060-2013; Mashinistov, Ruslan/M-8356-2015; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Aguilar Saavedra, Juan Antonio/F-1256-2016; Wemans, Andre/A-6738-2012; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Pacheco Pages, Andres/C-5353-2011; Riu, Imma/L-7385-2014; Cabrera Urban, Susana/H-1376-2015; Della Pietra, Massimo/J-5008-2012; Cavalli-Sforza, Matteo/H-7102-2015; Negrini, Matteo/C-8906-2014; Ferrer, Antonio/H-2942-2015; Hansen, John/B-9058-2015; Grancagnolo, Sergio/J-3957-2015; spagnolo, stefania/A-6359-2012; Shmeleva, Alevtina/M-6199-2015; Camarri, Paolo/M-7979-2015; Gavrilenko, Igor/M-8260-2015; Tikhomirov, Vladimir/M-6194-2015; Amorim, Antonio/C-8460-2013; Vanyashin, Aleksandr/H-7796-2013; Ferrando, James/A-9192-2012; Casadei, Diego/I-1785-2013; La Rosa, Alessandro/I-1856-2013; Moraes, Arthur/F-6478-2010; Smirnov, Sergei/F-1014-2011; Conde Muino, Patricia/F-7696-2011; Andreazza, Attilio/E-5642-2011; Boyko, Igor/J-3659-2013; Kuleshov, Sergey/D-9940-2013; Anjos, Nuno/I-3918-2013; Moorhead, Gareth/B-6634-2009; Ma, Hong/F-2725-2011; Gordon, Howard/D-6734-2013; Rud, Vyacheslav/D-6838-2012; Alexa, Calin/F-6345-2010; Orlov, Ilya/E-6611-2012; Petrucci, Fabrizio/G-8348-2012; Annovi, Alberto/G-6028-2012; Brooks, William/C-8636-2013; Stoicea, Gabriel/B-6717-2011; Fazio, Salvatore /G-5156-2010; Doyle, Anthony/C-5889-2009; Pina, Joao /C-4391-2012; Svatos, Michal/G-8437-2014; Chudoba, Jiri/G-7737-2014; Peleganchuk, Sergey/J-6722-2014; Santamarina Rios, Cibran/K-4686-2014; Bosman, Martine/J-9917-2014; Demirkoz, Bilge/C-8179-2014; Gutierrez, Phillip/C-1161-2011; Ventura, Andrea/A-9544-2015; Livan, Michele/D-7531-2012; Mitsou, Vasiliki/D-1967-2009; Joergensen, Morten/E-6847-2015; Mir, Lluisa-Maria/G-7212-2015; Smirnova, Oxana/A-4401-2013; Fabbri, Laura/H-3442-2012; Villa, Mauro/C-9883-2009; Kepka, Oldrich/G-6375-2014; Nemecek, Stanislav/G-5931-2014; Jakoubek, Tomas/G-8644-2014; Lokajicek, Milos/G-7800-2014; Staroba, Pavel/G-8850-2014; Kupco, Alexander/G-9713-2014; Mikestikova, Marcela/H-1996-2014; Kuday, Sinan/C-8528-2014; Snesarev, Andrey/H-5090-2013; Tomasek, Lukas/G-6370-2014 OI Monzani, Simone/0000-0002-0479-2207; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Olshevskiy, Alexander/0000-0002-8902-1793; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Maneira, Jose/0000-0002-3222-2738; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Gauzzi, Paolo/0000-0003-4841-5822; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Prokoshin, Fedor/0000-0001-6389-5399; Solfaroli Camillocci, Elena/0000-0002-5347-7764; Wolters, Helmut/0000-0002-9588-1773; Warburton, Andreas/0000-0002-2298-7315; De, Kaushik/0000-0002-5647-4489; Lee, Jason/0000-0002-2153-1519; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; Carvalho, Joao/0000-0002-3015-7821; Mashinistov, Ruslan/0000-0001-7925-4676; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Wemans, Andre/0000-0002-9669-9500; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Pacheco Pages, Andres/0000-0001-8210-1734; Riu, Imma/0000-0002-3742-4582; Della Pietra, Massimo/0000-0003-4446-3368; Negrini, Matteo/0000-0003-0101-6963; Ferrer, Antonio/0000-0003-0532-711X; Hansen, John/0000-0002-8422-5543; Grancagnolo, Sergio/0000-0001-8490-8304; spagnolo, stefania/0000-0001-7482-6348; Camarri, Paolo/0000-0002-5732-5645; Tikhomirov, Vladimir/0000-0002-9634-0581; Vanyashin, Aleksandr/0000-0002-0367-5666; Ferrando, James/0000-0002-1007-7816; La Rosa, Alessandro/0000-0001-6291-2142; Moraes, Arthur/0000-0002-5157-5686; Smirnov, Sergei/0000-0002-6778-073X; Conde Muino, Patricia/0000-0002-9187-7478; Andreazza, Attilio/0000-0001-5161-5759; Boyko, Igor/0000-0002-3355-4662; Kuleshov, Sergey/0000-0002-3065-326X; Moorhead, Gareth/0000-0002-9299-9549; Orlov, Ilya/0000-0003-4073-0326; Petrucci, Fabrizio/0000-0002-5278-2206; Annovi, Alberto/0000-0002-4649-4398; Brooks, William/0000-0001-6161-3570; Stoicea, Gabriel/0000-0002-7511-4614; Doyle, Anthony/0000-0001-6322-6195; Pina, Joao /0000-0001-8959-5044; Svatos, Michal/0000-0002-7199-3383; Peleganchuk, Sergey/0000-0003-0907-7592; Santamarina Rios, Cibran/0000-0002-9810-1816; Bosman, Martine/0000-0002-7290-643X; Ventura, Andrea/0000-0002-3368-3413; Livan, Michele/0000-0002-5877-0062; Mitsou, Vasiliki/0000-0002-1533-8886; Joergensen, Morten/0000-0002-6790-9361; Mir, Lluisa-Maria/0000-0002-4276-715X; Smirnova, Oxana/0000-0003-2517-531X; Fabbri, Laura/0000-0002-4002-8353; Villa, Mauro/0000-0002-9181-8048; Mikestikova, Marcela/0000-0003-1277-2596; Kuday, Sinan/0000-0002-0116-5494; Tomasek, Lukas/0000-0002-5224-1936 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union; ERC, European Union; NSRF, European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; NSRF, Greece; ISF, Israel; MINERVA, Israel; GIF, Israel; DIP, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; BRF, Norway; RCN, Norway; MNiSW, Poland; GRICES, Portugal; FCT, Portugal; MERYS (MECTS), Romania; MES of Russia, Russian Federation; ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MVZT, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET, ERC and NSRF, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT and NSRF, Greece; ISF, MINERVA, GIF, DIP and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; BRF and RCN, Norway; MNiSW, Poland; GRICES and FCT, Portugal; MERYS (MECTS), Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MVZT, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. NR 70 TC 12 Z9 12 U1 7 U2 148 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JAN PY 2013 IS 1 AR 029 DI 10.1007/JHEP01(2013)029 PG 46 WC Physics, Particles & Fields SC Physics GA 098XU UT WOS:000315583200029 ER PT J AU Altmannshofer, W Carena, M Shah, NR Yu, F AF Altmannshofer, Wolfgang Carena, Marcelo Shah, Nausheen R. Yu, Felix TI Indirect probes of the MSSM after the Higgs discovery SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Supersymmetry Phenomenology ID LARGE TAN-BETA; MINIMAL FLAVOR VIOLATION; SUPERSYMMETRIC THRESHOLD CORRECTIONS; ELECTROWEAK SYMMETRY-BREAKING; MISSING TRANSVERSE ENERGY; TOP-QUARK MASS; STANDARD MODEL; ATLAS DETECTOR; PP COLLISIONS; ROOT-S=7 TEV AB We study the minimal supersymmetric standard model (MSSM) with minimal flavor violation (MFV), imposing constraints from flavor physics observables and MSSM Higgs searches, in light of the recent discovery of a 125 GeV Higgs boson by ATLAS and CMS. We analyze the electroweak vacuum stability conditions to further restrict the MSSM parameter space. In addition, a connection to ultraviolet physics is shown via an implementation of renormalization group running, which determines the TeV-scale spectrum from a small set of minimal supergravity parameters. Finally, we investigate the impact from dark matter direct detection searches. Our work highlights the complementarity of collider, flavor and dark matter probes in exploring the MSSM, and shows that even in a MFV framework, flavor observables constrain the MSSM parameter space well beyond the current reach of direct SUSY particle searches. C1 [Altmannshofer, Wolfgang; Carena, Marcelo; Yu, Felix] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Carena, Marcelo] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carena, Marcelo] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Shah, Nausheen R.] Univ Michigan, Dept Phys, Michigan Ctr Theoret Phys, Ann Arbor, MI 48109 USA. RP Altmannshofer, W (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. EM waltmann@fnal.gov; carena@fnal.gov; naushah@umich.edu; felixyu@fnal.gov FU National Science Foundation [PHY-1066293]; INFN; United States Department of Energy [De-AC02-07CH11359]; DoE [DE-SC0007859] FX We would like to acknowledge helpful discussions with Stefania Gori, Arjun Menon and Carlos Wagner. We thank the Aspen Center for Physics for warm hospitality where part of this work was completed. The Aspen Center for Physics is supported by the National Science Foundation Grant No. PHY-1066293. W.A. thanks the Galileo Galilei Institute for Theoretical Physics for warm hospitality and the INFN for partial support during the completion of this work. Fermilab is operated by Fermi Research Alliance, LLC under Contract No. De-AC02-07CH11359 with the United States Department of Energy. N.R.S is supported by the DoE grant No. DE-SC0007859. NR 212 TC 51 Z9 51 U1 1 U2 4 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JAN PY 2013 IS 1 AR 160 DI 10.1007/JHEP01(2013)160 PG 52 WC Physics, Particles & Fields SC Physics GA 098XY UT WOS:000315583600079 ER PT J AU Batell, B Gori, S Wang, LT AF Batell, Brian Gori, Stefania Wang, Lian-Tao TI Higgs couplings and precision electroweak data SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Higgs Physics; LEP HERA and SLC Physics; Beyond Standard Model ID STANDARD MODEL; BOSON; LHC; DISCOVERY; RESONANCE; PHYSICS; SEARCH AB In light of the discovery of a Higgs-like particle at the LHC, we revisit the status of the precision electroweak data, focusing on two discrepant observables: 1) the long-standing 2.4 sigma deviation in the forward-backward asymmetry of the bottom quark A(FB)(b) , and 2) the 2.3 sigma deviation in R-b, the ratio of the Z -> b (b) over bar partial width to the inclusive hadronic width, which is now in tension after a recent calculation including new two-loop electroweak corrections. We consider possible resolutions of these discrepancies. Taking the data at face value, the most compelling scenario is that new physics directly affects A(FB)(b) and R-b, bringing the prediction into accord with the measured values. We propose a modified 'Beautiful Mirrors' scenario which contains new vector-like quarks that mix with the b quark, modifying the Zb (b) over bar vertex and thus correcting A(FB)(b) and R-b. We show that this scenario can lead to modifications to the production rates of the Higgs boson in certain channels, and in particular a sizable enhancement in the diphoton channel. We also describe additional collider tests of this scenario. C1 [Batell, Brian; Gori, Stefania; Wang, Lian-Tao] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Batell, Brian; Gori, Stefania; Wang, Lian-Tao] Univ Chicago, Dept Phys, Chicago, IL 60637 USA. [Gori, Stefania] Argonne Natl Lab, HEP Div, Argonne, IL 60439 USA. [Wang, Lian-Tao] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. RP Batell, B (reprint author), Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. EM batell@uchicago.edu; goris@uchicago.edu; liantaow@uchicago.edu FU U.S. Department of Energy (DOE), Div. of HEP [DE-AC02-06CH11357]; NSF [PHY-0756966]; DOE [DE-SC0003930]; DOE at the University of Washington [DE-FG02-96ER40956] FX We thank Ayres Freitas, Paul Langacker, and Carlos Wagner for helpful discussions and correspondence. S. G. and L. T. W. thank the Aspen Center of Physics where part of this work was completed. Work at ANL is supported in part by the U.S. Department of Energy (DOE), Div. of HEP, Contract DE-AC02-06CH11357. L. T. W. and B. B. are supported by the NSF under grant PHY-0756966 and the DOE Early Career Award under grant DE-SC0003930. B. B. was supported in part by the DOE under under Task TeV of contract DE-FG02-96ER40956 during the New Physics in Heavy Flavor in Hadron Colliders at the University of Washington. NR 104 TC 47 Z9 47 U1 0 U2 3 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JAN PY 2013 IS 1 AR 139 DI 10.1007/JHEP01(2013)139 PG 26 WC Physics, Particles & Fields SC Physics GA 098XY UT WOS:000315583600058 ER PT J AU Berger, J Stasto, AM AF Berger, J. Stasto, A. M. TI Exclusive vector meson production and small-x evolution SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Deep Inelastic Scattering (Phenomenology) ID DIFFRACTIVE ELECTROPRODUCTION; IMPACT PARAMETER; J/PSI MESONS; HERA; SCATTERING; QCD; LEPTOPRODUCTION; POMERON; RHO AB The process of exclusive elastic vector meson production in deep inelastic scattering is investigated within the dipole model framework supplemented by the small x evolution. The dipole-proton amplitude is obtained from the nonlinear Balitsky-Kovchegov evolution equation with impact parameter dependence. This dipole amplitude is used to compute the differential cross section for exclusive production of J/Psi, phi, and rho vector mesons. These numerical calculations are compared with the wide range of experimental data from HERA. Good agreement between the experimental data and the calculations is found. C1 [Berger, J.; Stasto, A. M.] Penn State Univ, University Pk, PA 16802 USA. [Stasto, A. M.] Brookhaven Natl Lab, RIKEN Ctr, Upton, NY 11793 USA. [Stasto, A. M.] Polish Acad Sci, H Niewodniczanski Inst Nucl Phys, Krakow, Poland. RP Berger, J (reprint author), Penn State Univ, University Pk, PA 16802 USA. EM jxb1024@psu.edu; astasto@phys.psu.edu FU Polish NCN [DEC-2011/01/B/ST2/03915]; DOE OJI [DE - SC0002145]; Sloan Foundation FX We thank Henri Kowalski for discussions as well as his assistance by allowing us usage of parts of his fortran code for the evaluation of the initial conditions. We also thank Emil Avsar and Mark Strikman for discussions. This work was supported by the Polish NCN grant DEC-2011/01/B/ST2/03915 and the DOE OJI grant No. DE - SC0002145. A.M.S. is supported by the Sloan Foundation. NR 39 TC 4 Z9 4 U1 1 U2 2 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. 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Swanson, J. CA CMS Collaboration TI Search for narrow resonances and quantum black holes in inclusive and b-tagged dijet mass spectra from pp collisions at root s=7 TeV SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering ID HADRON COLLIDERS; PHENOMENOLOGY; HIERARCHY AB A search for narrow resonances and quantum black holes is performed in inclusive and b-tagged dijet mass spectra measured with the CMS detector at the LHC. The data set corresponds to 5 fb(-1) of integrated luminosity collected in pp collisions at root s = 7 TeV. No narrow resonances or quantum black holes are observed. Model-independent upper limits at the 95% confidence level are obtained on the product of the cross section, branching fraction into dijets, and acceptance for three scenarios: decay into quark-quark, quark-gluon, and gluon-gluon pairs. Specific lower limits are set on the mass of string resonances (4.31 TeV), excited quarks (3.32 TeV), axigluons and colorons (3.36 TeV), scalar color-octet resonances (2.07 TeV), E-6 diquarks (3.75 TeV), and on the masses of W' (1.92 TeV) and Z' (1.47 TeV) bosons. The limits on the minimum mass of quantum black holes range from 4 to 5.3 TeV. In addition, b-quark tagging is applied to the two leading jets and upper limits are set on the production of narrow dijet resonances in a model-independent fashion as a function of the branching fraction to b-jet pairs. C1 [Chatrchyan, S.; Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Tumasyan, A.; Adam, W.; Aguilo, E.; Bergauer, T.; Dragicevic, M.; Eroe, J.; Fabjan, C.; Friedl, M.; Fruehwirth, R.; Ghete, V. 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M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Meneghelli, M.; Montanari, A.; Navarria, F. L.; Odorici, F.; Perrotta, A.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Abbiendi, G.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Capiluppi, P.; Castro, A.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Meneghelli, M.; Navarria, F. L.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gallo, E.; Gonzi, S.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gonzi, S.; Tropiano, A.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Colafranceschi, S.; Fabbri, F.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Fabbricatore, P.; Musenich, R.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Tosi, S.] Univ Genoa, Genoa, Italy. [Benaglia, A.; De Guio, F.; Di Matteo, L.; Fiorendi, S.; Gennai, S.; Ghezzi, A.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Massironi, A.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] Ist Nazl Fis Nucl, Sez Milano Bicocca, I-20133 Milan, Italy. [De Guio, F.; Di Matteo, L.; Fiorendi, S.; Ghezzi, A.; Manzoni, R. 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[Kanishchev, K.; Lazzizzera, I.] Univ Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Torre, P.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Torre, P.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Nappi, A.; Romeo, F.; Saha, A.; Santocchia, A.; Spiezia, A.; Taroni, S.; Pioppi, M.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Biasini, M.; Fano, L.; Lariccia, P.; Mantovani, G.; Nappi, A.; Romeo, F.; Santocchia, A.; Spiezia, A.; Taroni, S.; Pioppi, M.] Univ Perugia, I-06100 Perugia, Italy. [Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; D'Agnolo, R. T.; Dell'Orso, R.; Fiori, F.; Foa, L.; Giassi, A.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. 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[Choi, M.; Kim, J. H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. S.; Kwon, E.; Lee, B.; Lee, J.; Lee, S.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Bilinskas, M. J.; Grigelionis, I.; Janulis, M.; Juodagalvis, A.] Vilnius State Univ, Vilnius, Lithuania. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-De la Cruz, I.; Lopez-Fernandez, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.; Reyes-Santos, M. A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Bell, A. J.; Butler, P. H.; Doesburg, R.; Reucroft, S.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Asghar, M. I.; Butt, J.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Wolszczak, W.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Almeida, N.; Bargassa, P.; David, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. 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M.; Wan, X.; Wang, M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Simili, E.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Karaman, T.; Karapinar, G.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, L. N.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Yildirim, E.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey. [Bahtiyar, H.; Barlas, E.; Cankocak, K.; Vardarli, F. I.; Yucel, M.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Kreczko, L.; Metson, S.; Newbold, D. M.; Nirunpong, K.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Worm, S. D.; Newbold, D. M.; Basso, L.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Jackson, J.; Kennedy, B. W.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Womersley, W. J.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Bainbridge, R.; Ball, G.; Beuselinck, R.; Buchmuller, O.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Kenzie, M.; Lyons, L.; Magnan, A-M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Seez, C.; Sharp, P.; Sparrow, A.; Stoye, M.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Eld, S. Wake Fi; Wardle, N.; Whyntie, T.] Univ London Imperial Coll Sci Technol & Med, London, England. [Chadwick, M.; Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Hatakeyama, K.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; St John, J.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Bhattacharya, S.; Christopher, G.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Segala, M.; Sinthuprasith, T.; Speer, T.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Caulfield, M.; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Dolen, J.; Erbacher, R.; Gardner, M.; Houtz, R.; Ko, W.; Kopecky, A.; Lander, R.; Mall, O.; Miceli, T.; Nelson, R.; Pellett, D.; Ricci-Tam, F.; Rutherford, B.; Searle, M.; Smith, J.; Squires, M.; Tripathi, M.; Sierra, R. Vasquez; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Felcini, M.; Andreev, V.; Cline, D.; Cousins, R.; Duris, J.; Erhan, S.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Rakness, G.; Schlein, P.; Traczyk, P.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Babb, J.; Clare, R.; Dinardo, M. E.; Ellison, J.; Gary, J. W.; Giordano, F.; Hanson, G.; Liu, H.; Long, O. R.; Luthra, A.; Nguyen, H.; Paramesvaran, S.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; Evans, D.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Macneill, I.; Mangano, B.; Padhi, S.; Palmer, C.; Petrucciani, G.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Urthwein, F. W.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bellan, R.; Campagnari, C.; D'Alfonso, M.; Flowers, K.; Geffert, P.; George, C.; Golf, F.; Incandela, J.; Justus, C.; Kalavase, P.; Kovalskyi, D.; Mccoll, N.; Ribnik, J.; Richman, J.; Stuart, D.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dias, F. A.; Dubinin, M.; Apresyan, A.; Bornheim, A.; Chen, Y.; DiMarco, E.; Duarte, J.; Gataullin, M.; Ma, Y.; Mott, A.; Newman, H. B.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Veverka, J.; Wilkinson, R.; Xie, S.; Yang, Y.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Liu, Y. F.; Paulini, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Eggert, N.; Gibbons, L. K.; Heltsley, B.; Hopkins, W.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Fisk, I.; Freeman, J.; Green, D.; Gutsche, O.; Hanlon, J.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Klima, B.; Leonidopoulos, C.; Linacre, J.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Mason, D.; McBride, P.; Mishra, K.; Newman-Holmes, C.; Prokofyev, O.; Sexton-Kennedy, E.; Spiegel, L.; Taylor, L.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Yang, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Chen, M.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Drozdetskiy, A.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Gartner, J.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Park, M.; Remington, R.; Rinkevicius, A.; Sellers, P.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Hewamanage, S.; Lebolo, L. M.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Gleyzer, S. V.; Haas, J.; Hagopian, S.; Hagopian, V.; Jenkins, M.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Vodopiyanov, I.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Bai, Y.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Callner, J.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Lacroix, F.; O'Brien, C.; Silkworth, C.; Strom, D.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Ozturk, S.; Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Dilsiz, K.; Duru, F.; Griffiths, S.; Merlo, J-P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Newsom, C. R.; Norbeck, E.; Ogul, H.; Onel, Y.; Ozok, F.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Giurgiu, G.; Gritsan, A. V.; Guo, Z. J.; Hu, G.; Maksimovic, P.; Swartz, M.; Whitbeck, A.] Johns Hopkins Univ, Baltimore, MD USA. [Sibille, J.; Baringer, P.; Bean, A.; Benelli, G.; Kenny, R. P., III; Murray, M.; Noonan, D.; Sanders, S.; Stringer, R.; Tinti, G.; Wood, J. S.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Bolton, T.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kirn, M.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Peterman, A.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Bauer, G.; Bendavid, J.; Busza, W.; Butz, E.; Cali, I. A.; Chan, M.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Kim, Y.; Klute, M.; Krajczar, K.; Levin, A.; Luckey, P. D.; Ma, T.; Nahn, S.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Rudolph, M.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Sung, K.; Velicanu, D.; Wenger, E. A.; Wolf, R.; Wyslouch, B.; Yilmaz, Y.; Yoon, A. S.; Zanetti, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; De Benedetti, A.; Franzoni, G.; Gude, A.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Sasseville, M.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Cremaldi, L. M.; Kroeger, R.; Perera, L.; Rahmat, R.; Sanders, D. A.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Eads, M.; Keller, J.; Kravchenko, I.; Lazo-Flores, J.; Malik, S.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Kumar, A.; Rappoccio, S.; Wan, Z.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Nash, D.; Orimoto, T.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Anastassov, A.; Hahn, K. A.; Kubik, A.; Lusito, L.; Mucia, N.; Odell, N.; Ofierzynski, R. A.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Berry, D.; Brinkerhoff, A.; Chan, K. M.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kolb, J.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Morse, D. M.; Pearson, T.; Planer, M.; Ruchti, R.; Slaunwhite, J.; Valls, N.; Wayne, M.; Wolf, M.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Bylsma, B.; Durkin, L. S.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Puigh, D.; Rodenburg, M.; Smith, G.; Vuosalo, C.; Williams, G.; Winer, B. L.] Ohio State Univ, Columbus, OH 43210 USA. [Berry, E.; Elmer, P.; Halyo, V.; Hebda, P.; Hegeman, J.; Hunt, A.; Jindal, P.; Koay, S. A.; Pegna, D. Lopes; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Raval, A.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zenz, S. C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Brownson, E.; Lopez, A.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA. [Alagoz, E.; Barnes, V. E.; Benedetti, D.; Bolla, G.; Bortoletto, D.; De Mattia, M.; Everett, A.; Hu, Z.; Jones, M.; Koybasi, O.; Kress, M.; Laasanen, A. T.; Leonardo, N.; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Marono, M. Vidal; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Guragain, S.; Parashar, N.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Boulahouache, C.; Ecklund, K. M.; Geurts, F. J. M.; Li, W.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; Chung, Y. S.; Covarelli, R.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Miner, D. C.; Vishnevskiy, D.; Zielinski, M.] Univ Rochester, Rochester, NY 14627 USA. [Bhatti, A.; Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Malik, S.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Lath, A.; Panwalkar, S.; Park, M.; Patel, R.; Rekovic, V.; Robles, J.; Rose, K.; Salur, S.; Schnetzer, S.; Seitz, C.; Somalwar, S.; Stone, R.; Thomas, S.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Cerizza, G.; Hollingsworth, M.; Spanier, S.; Yang, Z. C.; York, A.] Univ Tennessee, Knoxville, TN USA. [Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Khotilovich, V.; Montalvo, R.; Osipenkov, I.; Pakhotin, Y.; Perloff, A.; Roe, J.; Safonov, A.; Sakuma, T.; Sengupta, S.; Suarez, I.; Tatarinov, A.; Toback, D.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Jeong, C.; Kovitanggoon, K.; Lee, S. W.; Libeiro, T.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Appelt, E.; Delannoy, A. G.; Florez, C.; Greene, S.; Gurrola, A.; Johns, W.; Kurt, P.; Maguire, C.; Melo, A.; Sharma, M.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN USA. [Arenton, M. W.; Balazs, M.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Lin, C.; Neu, C.; Wood, J.] Univ Virginia, Charlottesville, VA USA. [Gollapinni, S.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sakharov, A.] Wayne State Univ, Detroit, MI USA. [Anderson, M.; Belknap, D. A.; Borrello, L.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Friis, E.; Gray, L.; Grogg, K. S.; Grothe, M.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Klukas, J.; Lanaro, A.; Lazaridis, C.; Loveless, R.; Mohapatra, A.; Mozer, M. U.; Ojalvo, I.; Palmonari, F.; Pierro, G. A.; Ross, I.; Savin, A.; Smith, W. H.; Swanson, J.] Univ Wisconsin, Madison, WI 53706 USA. [Fabjan, C.; Fruehwirth, R.; Jeitler, M.; Krammer, M.; Wulz, C-E.] Vienna Univ Technol, A-1040 Vienna, Austria. 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RI Gulmez, Erhan/P-9518-2015; Seixas, Joao/F-5441-2013; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Ruiz, Alberto/E-4473-2011; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Rovelli, Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Leonidov, Andrey/M-4440-2013; Andreev, Vladimir/M-8665-2015; TUVE', Cristina/P-3933-2015; KIM, Tae Jeong/P-7848-2015; Arce, Pedro/L-1268-2014; Flix, Josep/G-5414-2012; Della Ricca, Giuseppe/B-6826-2013; Azarkin, Maxim/N-2578-2015; Paganoni, Marco/A-4235-2016; Kirakosyan, Martin/N-2701-2015; Lazzizzera, Ignazio/E-9678-2015; Sen, Sercan/C-6473-2014; D'Alessandro, Raffaello/F-5897-2015; Belyaev, Alexander/F-6637-2015; Stahl, Achim/E-8846-2011; Trocsanyi, Zoltan/A-5598-2009; Konecki, Marcin/G-4164-2015; Hernandez Calama, Jose Maria/H-9127-2015; Bedoya, Cristina/K-8066-2014; My, Salvatore/I-5160-2015; Matorras, Francisco/I-4983-2015; Ragazzi, Stefano/D-2463-2009; de la Cruz, Begona/K-7552-2014; Scodellaro, Luca/K-9091-2014; Josa, Isabel/K-5184-2014; Calvo Alamillo, Enrique/L-1203-2014; Paulini, Manfred/N-7794-2014; Vogel, Helmut/N-8882-2014; Marinho, Franciole/N-8101-2014; Ferguson, Thomas/O-3444-2014; Benussi, Luigi/O-9684-2014; Leonidov, Andrey/P-3197-2014; Dahms, Torsten/A-8453-2015; Grandi, Claudio/B-5654-2015; Bernardes, Cesar Augusto/D-2408-2015; Wolszczak, Weronika/N-3113-2013; Marlow, Daniel/C-9132-2014; de Jesus Damiao, Dilson/G-6218-2012; Janssen, Xavier/E-1915-2013; Bartalini, Paolo/E-2512-2014; Alves, Gilvan/C-4007-2013; Ligabue, Franco/F-3432-2014; Codispoti, Giuseppe/F-6574-2014; Gunaydin, Yusuf/F-7300-2014; Gribushin, Andrei/J-4225-2012; Cerrada, Marcos/J-6934-2014; Calderon, Alicia/K-3658-2014; Mundim, Luiz/A-1291-2012; Kodolova, Olga/D-7158-2012; Ivanov, Andrew/A-7982-2013; Hill, Christopher/B-5371-2012; Liu, Sheng/K-2815-2013; Zhukov, Valery/K-3615-2013; Venturi, Andrea/J-1877-2012; Manganote, Edmilson/K-8251-2013; Wimpenny, Stephen/K-8848-2013; Markina, Anastasia/E-3390-2012; Dudko, Lev/D-7127-2012; Dogangun, Oktay/L-9252-2013; Lokhtin, Igor/D-7004-2012; Novaes, Sergio/D-3532-2012; VARDARLI, Fuat Ilkehan/B-6360-2013; Wulz, Claudia-Elisabeth/H-5657-2011; Fruhwirth, Rudolf/H-2529-2012; Tinoco Mendes, Andre David/D-4314-2011; Rolandi, Luigi (Gigi)/E-8563-2013; Montanari, Alessandro/J-2420-2012; Petrushanko, Sergey/D-6880-2012; Raidal, Martti/F-4436-2012; Tomei, Thiago/E-7091-2012; Zalewski, Piotr/H-7335-2013 OI Gulmez, Erhan/0000-0002-6353-518X; Seixas, Joao/0000-0002-7531-0842; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Rovelli, Tiziano/0000-0002-9746-4842; TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; Arce, Pedro/0000-0003-3009-0484; Flix, Josep/0000-0003-2688-8047; Della Ricca, Giuseppe/0000-0003-2831-6982; Paganoni, Marco/0000-0003-2461-275X; Heath, Helen/0000-0001-6576-9740; Lazzizzera, Ignazio/0000-0001-5092-7531; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Belyaev, Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279; Konecki, Marcin/0000-0001-9482-4841; Hernandez Calama, Jose Maria/0000-0001-6436-7547; Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680; Matorras, Francisco/0000-0003-4295-5668; Ragazzi, Stefano/0000-0001-8219-2074; Scodellaro, Luca/0000-0002-4974-8330; Calvo Alamillo, Enrique/0000-0002-1100-2963; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Marinho, Franciole/0000-0002-7327-0349; Ferguson, Thomas/0000-0001-5822-3731; Benussi, Luigi/0000-0002-2363-8889; Dahms, Torsten/0000-0003-4274-5476; Grandi, Claudio/0000-0001-5998-3070; de Jesus Damiao, Dilson/0000-0002-3769-1680; Ligabue, Franco/0000-0002-1549-7107; Codispoti, Giuseppe/0000-0003-0217-7021; Gunaydin, Yusuf/0000-0002-0514-6936; Cerrada, Marcos/0000-0003-0112-1691; Mundim, Luiz/0000-0001-9964-7805; Ivanov, Andrew/0000-0002-9270-5643; Hill, Christopher/0000-0003-0059-0779; Wimpenny, Stephen/0000-0003-0505-4908; Dudko, Lev/0000-0002-4462-3192; Dogangun, Oktay/0000-0002-1255-2211; Novaes, Sergio/0000-0003-0471-8549; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Tinoco Mendes, Andre David/0000-0001-5854-7699; Rolandi, Luigi (Gigi)/0000-0002-0635-274X; Montanari, Alessandro/0000-0003-2748-6373; Tomei, Thiago/0000-0002-1809-5226; FU BMWF (Austria); FWF (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MES (Bulgaria); CERN (China); CAS (China); MoST (China); NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); MoER [SF0690030s09]; ERDF (Estonia); Academy of Finland (Finland); MEC (Finland); HIP (Finland); CEA (France); CNRS/IN2P3 (France); BMBF (Germany); DFG (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NKTH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF (Korea); WCU (Korea); LAS (Lithuania); CINVESTAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); MST (New Zealand); PAEC (Pakistan); MSHE (Poland); NSC (Poland); FCT (Portugal); JINR (Armenia); JINR (Belarus); JINR (Georgia); JINR (Ukraine); JINR (Uzbekistan); MON (Russia); RosAtom (Russia); RAS (Russia); RFBr (Russia); MSTD (Serbia); SEIDI (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); TUBITAK (Turkey); TAEK (Turkey); STFC (United Kingdom); DOE (U.S.A.); NSF (U.S.A.) FX We thank Can Kilic for calculations of the string resonance cross section, Ian Lewis for calculations of the S8 model cross section, and Bogdan Dobrescu for assistance in implementing the S8b model. We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC machine. We thank the technical and administrative staff at CERN and other CMS institutes, and acknowledge support from: BMWF and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); MoER, SF0690030s09 and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NKTH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF and WCU (Korea); LAS (Lithuania); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MST (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Armenia, Belarus, Georgia, Ukraine, Uzbekistan); MON, RosAtom, RAS and RFBr (Russia); MSTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); TUBITAK and TAEK (Turkey); STFC (United Kingdom); DOE and NSF (U.S.A.). NR 48 TC 7 Z9 7 U1 5 U2 109 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JAN PY 2013 IS 1 AR 013 DI 10.1007/JHEP01(2013)013 PG 40 WC Physics, Particles & Fields SC Physics GA 098XU UT WOS:000315583200013 ER PT J AU Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Aguilo, E Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hammer, J Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Pernicka, M Rahbaran, B Rohringer, C Rohringer, H Schofbeck, R Strauss, J Taurok, A Waltenberger, W Walzel, G Widl, E Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Bansal, M Bansal, S Cornelis, T De Wolf, EA Janssen, X Luyckx, S Mucibello, L Ochesanu, S Roland, B Rougny, R Selvaggi, M Staykova, Z Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Suarez, RG Kalogeropoulos, A Maes, M Olbrechts, A Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Clerbaux, B De Lentdecker, G Dero, V Gay, APR Hreus, T Leonard, A Marage, PE Mohammadi, A Reis, T Thomas, L Vander Marcken, G Vander Velde, C Vanlaer, P Wang, J Adler, V Beernaert, K Cimmino, A Costantini, S Garcia, G Grunewald, M Klein, B Lellouch, J Marinov, A Mccartin, J Rios, AAO Ryckbosch, D Strobbe, N Thyssen, F Tytgat, M Verwilligen, P Walsh, S Yazgan, E Zaganidis, N Basegmez, S Bruno, G Castello, R Ceard, L Delaere, C du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Lemaitre, V Liao, J Militaru, O Nuttens, C Pagano, D Pin, A Piotrzkowski, K Schul, N Garcia, JMV Beliy, N Caebergs, T Daubie, E Hammad, GH Alves, GA Martins, MC Damiao, DD Martins, T Pol, ME Souza, MHG Alda, WL Carvalho, W Custodio, A Da Costa, EM Martins, CD De Souza, SF Figueiredo, DM Mundim, L Nogima, H Oguri, V Da Silva, WLP Santoro, A Jorge, LS Sznajder, A Anjos, TS Bernardes, CA Dias, FA Tomei, TRFP Gregores, EM Lagana, C Marinho, F Mercadante, PC Novaes, SF Padula, SS Genchev, V Iaydjiev, P Piperov, S Rodozov, M Stoykova, S Sultanov, G Tcholakov, V Trayanov, R Vutova, M Dimitrov, A Hadjiiska, R Kozhuharov, V Litov, L Pavlov, B Petkov, P Bian, JG Chen, GM Chen, HS Jiang, CH Liang, D Liang, S Meng, X Tao, J Wang, J Wang, X Wang, Z Xiao, H Xu, M Zang, J Zhang, Z Asawatangtrakuldee, C Ban, Y Guo, Y Li, W Liu, S Mao, Y Qian, SJ Teng, H Wang, D Zhang, L Zou, W Avila, C Gomez, JP Moreno, BG Oliveros, AFO Sanabria, JC Godinovic, N Lelas, D Plestina, R Polic, D Puljak, I Antunovic, Z Kovac, M Brigljevic, V Duric, S Kadija, K Luetic, J Morovic, S Attikis, A Galanti, M Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Finger, M Finger, M Assran, Y Elgammal, S Kamel, AE Mahmoud, MA Radi, A Kadastik, M Muntel, M Raidal, M Rebane, L Tiko, A Eerola, P Fedi, G Voutilainen, M Harkonen, J Heikkinen, A Karimaki, V Kinnunen, R Kortelainen, MJ Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E Ungaro, D Wendland, L Banzuzi, K Karjalainen, A Korpela, A Tuuva, T Besancon, M Choudhury, S Dejardin, M Denegri, D Fabbro, B Faure, JL Ferri, F Ganjour, S Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Malcles, J Millischer, L Nayak, A Rander, J Rosowsky, A Shreyber, I Titov, M Baffioni, S Beaudette, F Benhabib, L Bianchini, L Bluj, M Broutin, C Busson, P Chariot, C Daci, N Dahms, T Dobrzynski, L de Cassagnac, RG Haguenauer, M Mine, P Mironov, C Naranjo, IN Nguyen, M Ochando, C Paganini, P Sabes, D Salerno, R Sirois, Y Veelken, C Zabi, A Agram, JL Andrea, J Bloch, D Bodin, D Brom, JM Cardaci, M Chabert, EC Collard, C Conte, E Drouhin, F Ferro, C Fontainem, JC Gele, D Goerlach, U Juillot, P Le Bihan, AC Van Hove, P Fassi, F Mercier, D Beauceron, S Beaupere, N Bondu, O Boudoul, G Chasserat, J Chierici, R Contardo, D Depasse, P El Mamouni, H Fay, J Gascon, S Gouzevitch, M Tile, B Kurca, T Lethuillier, M Mirabito, L Perries, S Sgandurra, L Sordini, V Tschudi, Y Verdier, P Viret, S Tsamalaidze, Z Anagnostou, G Autermann, C Beranek, S Edelhoff, M Feld, L Heracleous, N Hindrichs, O Jussen, R 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Melzer-Pellmann, IA Meyer, AB Mnich, J Mussgiller, A Naumann-Emme, S Novgorodova, O Olzem, J Perrey, H Petrukhin, A Pitzl, D Raspereza, A Cipriano, PMR Riedl, C Ron, E Rosin, M Salfeld-Nebgen, J Schmidt, R Schoerner-Sadenius, T Sen, N Spiridonov, A Stein, M Walsh, R Wissing, C Blobel, V Draeger, J Enderle, H Erfle, J Gebbert, U Gorner, M Hermanns, T Hoing, RS Kaschube, K Kaussen, G Kirschenmann, H Klanner, R Lange, J Mura, B Nowak, F Peiffer, T Pietsch, N Rathjens, D Sander, C Schettler, H Schleper, P Schlieckau, E Schmidt, A Schroder, M Schum, T Seidel, M Sola, V Stadie, H Steinbruck, G Thomsen, J Vanelderen, L Barth, C Berger, J Boser, C Chwalek, T De Boer, W Descroix, A Dierlamm, A Feindt, M Guthoff, M Hackstein, C Hartmann, F Hauth, T Heinrich, M Held, H Hoffmann, KH Husemann, U Katkov, I Komaragiri, JR Pardo, PL Martschei, D Mueller, S Muller, T Niegel, M Nurnberg, A Oberst, O Oehler, A Ott, J Quast, G Rabbertz, K Ratnikov, F Ratnikova, N Rocker, S Schilling, FP Schott, G Simonis, 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CA CMS collaboration TI Search for supersymmetry in final states with missing transverse energy and 0, 1, 2, or >= 3 b-quark jets in 7 TeV pp collisions using the variable alpha(T) SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering ID PROTON-PROTON COLLISIONS; ATLAS DETECTOR; GRAND UNIFICATION; STANDARD MODEL; SUPERGRAVITY; MOMENTUM; PARTICLE; SQUARKS; PHYSICS; SU(5) AB A search for supersymmetry in final states with jets and missing transverse energy is performed in pp collisions at a centre-of-mass energy of root s = 7 TeV. The data sample corresponds to an integrated luminosity of 4.98 fb(-1) collected by the CMS experiment at the LHC. In this search, a dimensionless kinematic variable, alpha(T), is used as the main discriminator between events with genuine and misreconstructed missing transverse energy. The search is performed in a signal region that is binned in the scalar sum of the transverse energy of jets and the number of jets identified as originating from a bottom quark. No excess of events over the standard model expectation is found. Exclusion limits are set in the parameter space of the constrained minimal supersymmetric extension of the standard model, and also in simplified models, with a special emphasis on compressed spectra and third-generation scenarios. C1 [Chatrchyan, S.; Khachatryan, V.; Sirunyan, A. M.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Aguilo, E.; Bergauer, T.; Dragicevic, M.; Eroe, J.; Fabjan, C.; Friedl, M.; Fruehwirth, R.; Ghete, V. M.; Hammer, J.; Hoermann, N.; Hrubec, J.; Jeitler, M.; Kiesenhofer, W.; Knuenz, V.; Krammer, M.; Kraetschmer, I.; Liko, D.; Mikulec, I.; Pernicka, M.; Rahbaran, B.; Rohringer, C.; Rohringer, H.; Schoefbeck, R.; Strauss, J.; Taurok, A.; Waltenberger, W.; Walzel, G.; Widl, E.; Wulz, C-E.] Inst Hochenergiephys OeAW, Vienna, Austria. [Mossolov, V.; Shumeiko, N.; Gonzalez, J. Suarez] Natl Ctr Particle & High Energy Phys, Minsk, Byelarus. [Bansal, M.; Bansal, S.; Cornelis, T.; De Wolf, E. A.; Janssen, X.; Luyckx, S.; Mucibello, L.; Ochesanu, S.; Roland, B.; Rougny, R.; Selvaggi, M.; Staykova, Z.; Van Haevermaet, H.; Van Mechelen, P.; Van Remortel, N.; Van Spilbeeck, A.] Univ Antwerp, B-2020 Antwerp, Belgium. [Blekman, F.; Blyweert, S.; D'Hondt, J.; Suarez, R. Gonzalez; Kalogeropoulos, A.; Maes, M.; Olbrechts, A.; Van Doninck, W.; Van Mulders, P.; Van Onsem, G. P.; Villella, I.] Vrije Univ Brussel, Brussels, Belgium. [Clerbaux, B.; De Lentdecker, G.; Dero, V.; Gay, A. P. R.; Hreus, T.; Leonard, A.; Marage, P. E.; Mohammadi, A.; Reis, T.; Thomas, L.; Vander Marcken, G.; Vander Velde, C.; Vanlaer, P.; Wang, J.] Univ Libre Bruxelles, Brussels, Belgium. [Adler, V.; Beernaert, K.; Cimmino, A.; Costantini, S.; Garcia, G.; Grunewald, M.; Klein, B.; Lellouch, J.; Marinov, A.; Mccartin, J.; Rios, A. A. Ocampo; Ryckbosch, D.; Strobbe, N.; Thyssen, F.; Tytgat, M.; Verwilligen, P.; Walsh, S.; Yazgan, E.; Zaganidis, N.] Univ Ghent, B-9000 Ghent, Belgium. [Basegmez, S.; Bruno, G.; Castello, R.; Ceard, L.; Delaere, C.; du Pree, T.; Favart, D.; Forthomme, L.; Giammanco, A.; Hollar, J.; Lemaitre, V.; Liao, J.; Militaru, O.; Nuttens, C.; Pagano, D.; Pin, A.; Piotrzkowski, K.; Schul, N.; Garcia, J. M. Vizan] Catholic Univ Louvain, B-1348 Louvain, Belgium. [Beliy, N.; Caebergs, T.; Daubie, E.; Hammad, G. H.] Univ Mons, B-7000 Mons, Belgium. [Alves, G. A.; Correa Martins Junior, M.; De Jesus Damiao, D.; Martins, T.; Pol, M. E.; Souza, M. H. G.] Ctr Brasileiro Pesquisas Fis, Rio De Janeiro, Brazil. [Alda Junior, W. L.; Carvalho, W.; Custodio, A.; Da Costa, E. M.; De Oliveira Martins, C.; Fonseca De Souza, S.; Matos Figueiredo, D.; Mundim, L.; Nogima, H.; Oguri, V.; Prado Da Silva, W. L.; Santoro, A.; Soares Jorge, L.; Sznajder, A.] Univ Estado Rio de Janeiro, BR-20550011 Rio De Janeiro, Brazil. [Anjos, T. S.; Bernardes, C. A.; Dias, F. A.; Fernandez Perez Tomei, T. R.; Gregores, E. M.; Lagana, C.; Marinho, F.; Mercadante, P. C.; Novaes, S. F.; Padula, Sandra S.] Univ Estadual Paulista, Inst Fis Teor, BR-01405 Sao Paulo, Brazil. [Genchev, V.; Iaydjiev, P.; Piperov, S.; Rodozov, M.; Stoykova, S.; Sultanov, G.; Tcholakov, V.; Trayanov, R.; Vutova, M.] Bulgarian Acad Sci, Inst Nucl Res & Nucl Energy, Sofia, Bulgaria. [Dimitrov, A.; Hadjiiska, R.; Kozhuharov, V.; Litov, L.; Pavlov, B.; Petkov, P.] Univ Sofia, BU-1126 Sofia, Bulgaria. [Bian, J. G.; Chen, G. M.; Chen, H. S.; Jiang, C. H.; Liang, D.; Liang, S.; Meng, X.; Tao, J.; Wang, J.; Wang, X.; Wang, Z.; Xiao, H.; Xu, M.; Zang, J.; Zhang, Z.] Inst High Energy Phys, Beijing 100039, Peoples R China. [Asawatangtrakuldee, C.; Ban, Y.; Guo, Y.; Li, W.; Liu, S.; Mao, Y.; Qian, S. J.; Teng, H.; Wang, D.; Zhang, L.; Zou, W.] Peking Univ, State Key Lab Nucl Phys & Tech, Beijing 100871, Peoples R China. [Avila, C.; Gomez, J. P.; Gomez Moreno, B.; Osorio Oliveros, A. F.; Sanabria, J. C.] Univ Los Andes, Bogota, Colombia. [Godinovic, N.; Lelas, D.; Plestina, R.; Polic, D.; Puljak, I.] Tech Univ Split, Split, Croatia. [Antunovic, Z.; Kovac, M.] Univ Split, Split, Croatia. [Brigljevic, V.; Duric, S.; Kadija, K.; Luetic, J.; Morovic, S.] Rudjer Boskovic Inst, Zagreb, Croatia. [Attikis, A.; Galanti, M.; Mavromanolakis, G.; Mousa, J.; Nicolaou, C.; Ptochos, F.; Razis, P. A.] Univ Cyprus, Nicosia, Cyprus. [Finger, M.; Finger, M., Jr.] Charles Univ Prague, Prague, Czech Republic. [Assran, Y.; Elgammal, S.; Kamel, A. Ellithi; Mahmoud, M. A.; Radi, A.] Acad Sci Res & Technol Arab Republ Egypt, Egyptian Network High Energy Phys, Cairo, Egypt. [Giammanco, A.; Kadastik, M.; Muentel, M.; Raidal, M.; Rebane, L.; Tiko, A.] NICPB, Tallinn, Estonia. [Eerola, P.; Fedi, G.; Voutilainen, M.] Univ Helsinki, Dept Phys, Helsinki, Finland. [Harkonen, J.; Heikkinen, A.; Karimaki, V.; Kinnunen, R.; Kortelainen, M. J.; Lampen, T.; Lassila-Perini, K.; Lehti, S.; Linden, T.; Luukka, P.; Maenpaa, T.; Peltola, T.; Tuominen, E.; Tuominiemi, J.; Tuovinen, E.; Ungaro, D.; Wendland, L.] Helsinki Inst Phys, Helsinki, Finland. [Banzuzi, K.; Karjalainen, A.; Korpela, A.; Tuuva, T.] Lappeenranta Univ Technol, Lappeenranta, Finland. [Besancon, M.; Choudhury, S.; Dejardin, M.; Denegri, D.; Fabbro, B.; Faure, J. L.; Ferri, F.; Ganjour, S.; Givernaud, A.; Gras, P.; de Monchenault, G. Hamel; Jarry, P.; Locci, E.; Malcles, J.; Millischer, L.; Nayak, A.; Rander, J.; Rosowsky, A.; Shreyber, I.; Titov, M.] CEA Saclay, DSM IRFU, F-91191 Gif Sur Yvette, France. [Plestina, R.; Baffioni, S.; Beaudette, F.; Benhabib, L.; Bianchini, L.; Bluj, M.; Broutin, C.; Busson, P.; Chariot, C.; Daci, N.; Dahms, T.; Dobrzynski, L.; de Cassagnac, R. Granier; Haguenauer, M.; Mine, P.; Mironov, C.; Naranjo, I. N.; Nguyen, M.; Ochando, C.; Paganini, P.; Sabes, D.; Salerno, R.; Sirois, Y.; Veelken, C.; Zabi, A.; Bernet, C.] Ecole Polytech, CNRS, IN2P3, Lab Leprince Ringuet, F-91128 Palaiseau, France. [Agram, J-L.; Andrea, J.; Bloch, D.; Bodin, D.; Brom, J-M.; Cardaci, M.; Chabert, E. C.; Collard, C.; Conte, E.; Drouhin, F.; Ferro, C.; Fontainem, J-C.; Gele, D.; Goerlach, U.; Juillot, P.; Le Bihan, A-C.; Van Hove, P.] Univ Haute Alsace Mulhouse, Univ Strasbourg, Inst Pluridisciplinaire Hubert Curien, CNRS,IN2P3, Strasbourg, France. [Fassi, F.; Mercier, D.] Inst Natl Phys Nucl & Phys Particules, Ctr Calcul, CNRS, IN2P3, Villeurbanne, France. [Beauceron, S.; Beaupere, N.; Bondu, O.; Boudoul, G.; Chasserat, J.; Chierici, R.; Contardo, D.; Depasse, P.; El Mamouni, H.; Fay, J.; Gascon, S.; Gouzevitch, M.; Tile, B.; Kurca, T.; Lethuillier, M.; Mirabito, L.; Perries, S.; Sgandurra, L.; Sordini, V.; Tschudi, Y.; Verdier, P.; Viret, S.] Univ Lyon 1, CNRS, IN2P3, Inst Phys Nucl Lyon, F-69622 Villeurbanne, France. [Tsamalaidze, Z.] Tbilisi State Univ, Inst High Energy Phys & Informatizat, GE-380086 Tbilisi, Rep of Georgia. [Anagnostou, G.; Autermann, C.; Beranek, S.; Edelhoff, M.; Feld, L.; Heracleous, N.; Hindrichs, O.; Jussen, R.; Klein, K.; Merz, J.; Ostapchuk, A.; Perieanu, A.; Raupach, F.; Sammet, J.; Schael, S.; Sprenger, D.; Weber, H.; Wittmer, B.; Zhukov, V.] Rhein Westfal TH Aachen, Inst Phys 1, Aachen, Germany. [Ata, M.; Caudron, J.; Dietz-Laursonn, E.; Duchardt, D.; Erdmann, M.; Fischer, R.; Gueth, A.; Hebbeker, T.; Heidemann, C.; Hoepfner, K.; Klingebiel, D.; Kreuzer, P.; Merschmeyer, M.; Meyer, A.; Olschewski, M.; Papacz, P.; Pieta, H.; Reithler, H.; Schmitz, S. A.; Sonnenschein, L.; Steggemann, J.; Teyssier, D.; Weber, M.] Rhein Westfal TH Aachen, Phys Inst A 3, Aachen, Germany. [Bontenackels, M.; Cherepanov, V.; Erdogan, Y.; Fluegge, G.; Geenen, H.; Geisler, M.; Ahmad, W. Haj; Hoehle, F.; Kargoll, B.; Kress, T.; Kuessel, Y.; Lingemann, J.; Nowack, A.; Perchalla, L.; Pooth, O.; Land, P. Sauer; Stahl, A.] Rhein Westfal TH Aachen, Phys Inst B 3, Aachen, Germany. [Martin, M. Aldaya; Behr, J.; Behrenhoff, W.; Behrens, U.; Bergholz, M.; Bethani, A.; Borras, K.; Burgmeier, A.; Cakir, A.; Calligaris, L.; Campbell, A.; Castro, E.; Costanza, F.; Dammann, D.; Pardos, C. Diez; Eckerlin, G.; Eckstein, D.; Flucke, G.; Geiser, A.; Glushkov, I.; Gunnellini, P.; Habib, S.; Hauk, J.; Hellwig, G.; Jung, H.; Kasemann, M.; Katsas, P.; Kleinwort, C.; Kluge, H.; Knutsson, A.; Kraemer, M.; Kruecker, D.; Kuznetsova, E.; Lange, W.; Lohmann, W.; Lutz, B.; Mankel, R.; Marfin, I.; Marienfeld, M.; Melzer-Pellmann, I-A.; Meyer, A. B.; Mnich, J.; Mussgiller, A.; Naumann-Emme, S.; Novgorodova, O.; Olzem, J.; Perrey, H.; Petrukhin, A.; Pitzl, D.; Raspereza, A.; Cipriano, P. M. Ribeiro; Riedl, C.; Ron, E.; Rosin, M.; Salfeld-Nebgen, J.; Schmidt, R.; Schoerner-Sadenius, T.; Sen, N.; Spiridonov, A.; Stein, M.; Walsh, R.; Wissing, C.] DESY, Hamburg, Germany. [Blobel, V.; Draeger, J.; Enderle, H.; Erfle, J.; Gebbert, U.; Goerner, M.; Hermanns, T.; Hoeing, R. S.; Kaschube, K.; Kaussen, G.; Kirschenmann, H.; Klanner, R.; Lange, J.; Mura, B.; Nowak, F.; Peiffer, T.; Pietsch, N.; Rathjens, D.; Sander, C.; Schettler, H.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Schroeder, M.; Schum, T.; Seidel, M.; Sola, V.; Stadie, H.; Steinbrueck, G.; Thomsen, J.; Vanelderen, L.] Univ Hamburg, Hamburg, Germany. [Barth, C.; Berger, J.; Boeser, C.; Chwalek, T.; De Boer, W.; Descroix, A.; Dierlamm, A.; Feindt, M.; Guthoff, M.; Hackstein, C.; Hartmann, F.; Hauth, T.; Heinrich, M.; Held, H.; Hoffmann, K. H.; Husemann, U.; Katkov, I.; Komaragiri, J. R.; Pardo, P. Lobelle; Martschei, D.; Mueller, S.; Mueller, Th.; Niegel, M.; Nuernberg, A.; Oberst, O.; Oehler, A.; Ott, J.; Quast, G.; Rabbertz, K.; Ratnikov, F.; Ratnikova, N.; Roecker, S.; Schilling, F-P.; Schott, G.; Simonis, H. J.; Stober, F. M.; Troendle, D.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weiler, T.; Zeise, M.] Univ Karlsruhe, Inst Expt Kernphys, Karlsruhe, Germany. [Daskalakis, G.; Geralis, T.; Kesisoglou, S.; Kyriakis, A.; Loukas, D.; Manolakos, I.; Markou, A.; Markou, C.; Mavrommatis, C.; Ntomari, E.] Inst Nucl Phys Demokritos, Aghia Paraskevi, Greece. [Gouskos, L.; Mertzimekis, T. J.; Panagiotou, A.; Saoulidou, N.; Cerci, S.; Cerci, D. Sunar; Tai, B.] Univ Athens, Athens, Greece. [Evangelou, I.; Foudas, C.; Kokkas, P.; Manthos, N.; Papadopoulos, I.; Patras, V.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Krajczar, K.] KFKI Res Inst Particle & Nucl Phys, Budapest, Hungary. [Horvath, D.; Beni, N.; Czellar, S.; Molnar, J.; Palinkas, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Karancsi, J.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, H-4012 Debrecen, Hungary. [Beri, S. B.; Bhatnagar, V.; Dhingra, N.; Gupta, R.; Kaur, M.; Mehta, M. Z.; Nishu, N.; Saini, L. K.; Sharma, A.; Singh, J. B.] Panjab Univ, Chandigarh 160014, India. [Kumar, Ashok; Kumar, Arun; Ahuja, S.; Bhardwaj, A.; Choudhary, B. C.; Malhotra, S.; Naimuddin, M.; Ranjan, K.; Sharma, V.; Shivpuri, R. K.] Univ Delhi, Delhi 110007, India. [Banerjee, S.; Bhattacharya, S.; Dutta, S.; Comber, B.; Jain, Sa; Jain, Sh; Khurana, R.; Sarkar, S.; Sharan, M.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Choudhury, R. K.; Dutta, D.; Kailas, S.; Kumar, V.; Mehta, P.; Mohanty, A. K.; Pant, L. M.; Shukla, P.] Bhabha Atom Res Ctr, Bombay 400085, Maharashtra, India. [Aziz, T.; Ganguly, S.; Guchait, M.; Maity, M.; Majumder, G.; Mazumdar, K.; Mohanty, G. B.; Panda, B.; Sudhakar, K.; Wickramage, N.] Tata Inst Fundamental Res EHEP, Bombay, Maharashtra, India. [Guchait, M.; Banerjee, S.; Dugad, S.] Tata Inst Fundamental Res HECR, Bombay, Maharashtra, India. [Arfaei, H.; Bakhshiansohi, H.; Etesami, S. M.; Fahim, A.; Hashemi, M.; Hesari, H.; Jafari, A.; Khakzad, M.; Najafabadi, M. Mohammadi; Mehdiabadi, S. Paktinat; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; Colaleo, A.; Creanza, D.; De Fiippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Lusito, L.; Maggi, G.; Maggi, M.; Marangelli, B.; My, S.; Nuzzo, S.; Pacifico, N.; Pompili, A.; Pugliese, G.; Selvaggi, G.; Slivestris, L.; Singh, G.; Venditti, R.; Zito, G.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; De Palma, M.; Lusito, L.; Marangelli, B.; Nuzzo, S.; Pacifico, N.; Pompili, A.; Selvaggi, G.; Singh, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Fiippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Benvenutia, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Capthippi, P.; Castro, A.; Cavallo, F. R.; Cufflani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Meneghelli, M.; Montanari, A.; Navarria, F. L.; Odorici, F.; Perrotta, A.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Travaglini, R.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Capthippi, P.; Castro, A.; Cufflani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Meneghelli, M.; Navarria, F. L.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gallo, E.; Goizi, S.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [D'Alessandro, R.; Focardi, E.; Frosali, S.; Goizi, S.; Tropiano, A.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Colafranceschi, S.; Fabbri, F.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Fabbricatore, P.; Musenich, R.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Tosi, S.] Univ Genoa, Genoa, Italy. [Benaglia, A.; De Guio, F.; Di Matteo, L.; Fiorendi, S.; Gennai, S.; Ghezzi, A.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Massironi, A.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; Sala, S.; de Fatis, T. Tabarelli] Ist Nazl Fis Nucl, Sez Milano Bicocca, I-20133 Milan, Italy. [Benaglia, A.; De Guio, F.; Di Matteo, L.; Fiorendi, S.; Ghezzi, A.; Manzoni, R. 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T.; Pazzini, J.; Ronchese, P.; Simonetto, F.; Vanini, S.; Zotto, P.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.; Lazzizzera, I.] Univ Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Torre, P.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Torre, P.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Nappi, A.; Romeo, F.; Saha, A.; Santocchia, A.; Spiezia, A.; Taroni, S.; Pioppi, M.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Biasini, M.; Fano, L.; Lariccia, P.; Mantovani, G.; Nappi, A.; Romeo, F.; Santocchia, A.; Spiezia, A.; Taroni, S.; Pioppi, M.] Univ Perugia, I-06100 Perugia, Italy. [Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; D'Agnolo, R. T.; Dell'Orso, R.; Fiori, F.; Foa, L.; Giassi, A.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. C.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Fiori, F.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Azzurri, P.; Broccolo, G.; D'Agnolo, R. T.; Foa, L.; Ligabue, F.; Rolandi, G.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Diemoz, M.; Fanelli, C.; Grassi, M.; Longo, E.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Sigamani, M.; Soffi, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; Del Re, D.; Fanelli, C.; Grassi, M.; Longo, E.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Soffi, L.; Potenza, A.; Romero, A.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Biino, C.; Cartiglia, N.; Costa, M.; Demaria, N.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Pastrone, N.; Pelliccioni, M.; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Pereira, A. Vilela] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Costa, M.; Migliore, E.; Monaco, V.; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; Marone, M.; Montanino, D.; Penzo, A.; Schizzi, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; Marone, M.; Montanino, D.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Heo, S. G.; Kim, T. Y.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Chang, S.; Kim, D. H.; Kim, G. N.; Kong, D. J.; Park, H.; Ro, S. R.; Son, D. C.; Son, T.; Kamon, T.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, J. Y.; Kim, Zero J.; Song, S.] Chonnam Natl Univ, Inst Univ & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, T. J.; Lee, K. S.; Moon, D. H.; Park, S. K.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Cho, Y.; Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. S.; Kwon, E.; Lee, B.; Lee, J.; Lee, S.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Bilinskas, M. J.; Grigelionis, I.; Janulis, M.; Juodagalvis, A.] Vilnius State Univ, Vilnius, Lithuania. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de la Cruz, I.; Lopez-Fernandez, R.; Villalba, R. Magana; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.; Reyes-Santos, M. A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Bell, A. J.; Butler, P. H.; Doesburg, R.; Reucroft, S.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Ansari, M. H.; Asghar, M. I.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bluj, M.; Bialkowska, H.; Boimska, B.; Frueboes, T.; Gokieli, R.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Almeida, N.; Bargassa, P.; David, A.; Faccioli, P.; Parracho, P. C. Ferreira; Gallinaro, M.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Tsamalaidze, Z.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Karjavin, V.; Konoplyanikov, V.; Kozlov, G.; Laney, A.; Malakhov, A.; Moisenz, P.; Palichik, V.; Perelygin, V.; Savina, M.; Shmatov, S.; Shulha, S.; Smirnov, V.; Volodko, A.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Evstyukhin, S.; Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Matveev, V.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Erofeeva, M.; Gavrilov, V.; Kossov, M.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Stolin, V.; Vlasov, E.; Zhokin, A.; Sibille, J.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Zhukov, V.; Katkov, I.; Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Markina, A.; Obraztsov, S.; Perfilov, M.; Petrushanko, S.; Popov, A.; Sarycheva, L.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Grishin, V.; Kachanov, V.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Maestre, J. Alcaraz; Arce, P.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Pelayo, J. Puerta; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.; Willmott, C.] CIEMAT, E-28040 Madrid, Spain. [Albajar, C.; Codispoti, G.; de Troconiz, J. F.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.; Piedra Gomez, J.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Chuang, S. H.; Duarte Campderros, J.; Felcini, M.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Graziano, A.; Jorda, C.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Genchev, V.; Iaydjiev, P.; Puljak, I.; Chierici, R.; Lingemann, J.; Guthoff, M.; Hauth, T.; Mohanty, A. K.; De Fiippis, N.; Fasanella, D.; Meneghelli, M.; Di Matteo, L.; Gennai, S.; Massironi, A.; De Cosa, A.; Paolucci, P.; Bacchetta, N.; Branca, A.; Nespolo, M.; D'Agnolo, R. T.; Fiori, F.; Squillacioti, P.; Grassi, M.; Meridiani, P.; Mariotti, C.; Musich, M.; Marone, M.; Montanino, D.; Grishin, V.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Perez, J. A. Coarasa; D'Enterria, D.; Dabrowski, A.; De Roeck, A.; Di Guida, S.; Dobson, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Frisch, B.; Funk, W.; Georgiou, G.; Giffels, M.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Giunta, M.; Glege, F.; Garrido, R. Gomez-Reino; Govoni, P.; Gowdy, S.; Guida, R.; Hansen, M.; Harris, P.; Hartl, C.; Harvey, J.; Hegner, B.; Hinzmann, A.; Innocente, V.; Janot, P.; Kaadze, K.; Karavakis, E.; Kousouris, K.; Lecoq, P.; Lee, Y-J.; Lenzi, P.; Lourenco, C.; Magini, N.; Maeki, T.; Malberti, M.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moser, R.; Mozer, M. U.; Mulders, M.; Musella, P.; Nesvold, E.; Orimoto, T.; Orsini, L.; Cortezon, E. Palencia; Perez, E.; Perrozzi, L.; Petrilli, A.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Piparo, D.; Polese, G.; Quertenmont, L.; Racz, A.; Reece, W.; Antunes, J. Rodrigues; Rolandi, G.; Rovelli, C.; Rovere, M.; Sakulin, H.; Santanastasio, F.; Schaefer, C.; Schwick, C.; Segoni, I.; Sekmen, S.; Sharma, A.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Tsirou, A.; Veres, G. I.; Vlimant, J. R.; Woehri, H. K.; Worm, S. D.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Worm, S. D.; Bertl, W.; Deiters, K.; Erdmann, W.; Gabathuler, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Meier, F.; Renker, D.; Rohe, T.; Sibille, J.; Newbold, D. M.] Paul Scherrer Inst, Villigen, Switzerland. [Baeni, L.; Bortignon, P.; Buchmann, M. A.; Casal, B.; Chanon, N.; Deisher, A.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eugster, J.; Freudenreich, K.; Grab, C.; Hits, D.; Lecomte, P.; Lustermann, W.; Marini, A. C.; Del Arbol, P. Martinez Ruiz; Mohr, N.; Moortgat, F.; Naegeli, C.; Nef, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pape, L.; Pauss, F.; Peruzzi, M.; Ronga, F. J.; Rossini, M.; Sala, L.; Sanchez, A. K.; Starodumov, A.; Stieger, B.; Takahashi, M.; Tauscher, L.; Thea, A.; Theofilatos, K.; Treille, D.; Urscheler, C.; Wallny, R.; Weber, H. A.; Wehrli, L.] ETH, Inst Particle Phys, Zurich, Switzerland. [Amsler, C.; Chiochia, V.; De Visscher, S.; Favaro, C.; Rikova, M. Ivova; Mejias, B. Millan; Otiougova, P.; Robmann, P.; Snoek, H.; Tupputi, S.; Verzetti, M.] Univ Zurich, Zurich, Switzerland. [Chang, Y. H.; Chen, K. H.; Kuo, C. M.; Li, S. W.; Lin, W.; Liu, Z. K.; Lu, Y. J.; Mekterovic, D.; Singh, A. P.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Dietz, C.; Grundler, U.; Hou, W-S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Lu, R-S.; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wan, X.; Wang, M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Srimanobhas, N.] Chulalongkorn Univ, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Karaman, T.; Karapinar, G.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tai, B.; Topakli, H.; Vergili, L. N.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Ler, A. M. Gu; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Yildirim, E.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey. [Cankocak, K.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Bostock, F.; Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Kreczko, L.; Lucas, C.; Meng, Z.; Metson, S.; Newbold, D. M.; Nirunpong, K.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Rovelli, C.; Basso, L.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Jackson, J.; Kennedy, B. W.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Womersley, W. J.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Bainbridge, R.; Ball, G.; Beuselinck, R.; Buchmuller, O.; Burton, D. L.; Ling, D. Col; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Lyons, L.; Magnan, A-M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Papageorgiou, A.; La, J. Pe; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Ryan, M. J.; Seez, C.; Sharp, P.; Sparrow, A.; Stoye, M.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.; Whyntie, T.] Univ London Imperial Coll Sci Technol & Med, London, England. [Chadwick, M.; Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Hatakeyama, K.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; St John, J.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Bhattacharya, S.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Nguyen, D.; La, M. Sega; Sinthuprasith, T.; Speer, T.; Tsang, K. V.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De la Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Do Len, J.; Erbacher, R.; Gardner, M.; Houtz, R.; Ko, W.; Kopecky, A.; Lander, R.; Mall, O.; Miceli, T.; Pellett, D.; Ricci-Tam, F.; Rutherford, B.; Searle, M.; Smith, J.; Squires, M.; Tripathi, M.; Sierra, R. Vasquez; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Felcini, M.; Andreev, V.; Cline, D.; Cousins, R.; Duris, J.; Erhan, S.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Plager, C.; Rakness, G.; Schlein, P.; Traczyk, P.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Babb, J.; Clare, R.; Dinardo, M. E.; Ellison, J.; Gary, J. W.; Giordano, F.; Hanson, G.; Jeng, G. Y.; Liu, H.; Long, O. R.; Luthra, A.; Nguyen, H.; Paramesvaran, S.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; Evans, D.; Golf, F.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Macneill, I.; Mangano, B.; Padhi, S.; Palmer, C.; Petrucciani, G.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bellan, R.; Campagnari, C.; D'Alfonso, M.; Danielson, T.; Flowers, K.; Geffert, P.; Incandela, J.; Justus, C.; Kalavase, P.; Koay, S. A.; Kovalskyi, D.; Krutelyov, V.; Lowette, S.; Mccoll, N.; Pavlunin, V.; Rebassoo, F.; Ribnik, J.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dias, F. A.; Dubinin, M.; Apresyan, A.; Bornheim, A.; Chen, Y.; Di Marco, E.; Duarte, J.; Gataullin, M.; Ma, Y.; Mott, A.; Newman, H. B.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Veverka, J.; Wilkinson, R.; Xie, S.; Yang, Y.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Akgun, B.; Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Liu, Y. F.; Paulini, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Eggert, N.; Gibbons, L. K.; Heltsley, B.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Vaughan, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bloch, I.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Green, D.; Gutsche, O.; Hanlon, J.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Kilminster, B.; Klima, B.; Kunori, S.; Kwan, S.; Leonidopoulos, C.; Linacre, J.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Wu, W.; Yang, F.; Yumiceva, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Chen, M.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Drozdetskiy, A.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Gartner, J.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Park, M.; Remington, R.; Rinkevicius, A.; Sellers, P.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Hewamanage, S.; Lebolo, L. M.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Gleyzer, S. V.; Haas, J.; Hagopian, S.; Hagopian, V.; Jenkins, M.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Vodopiyanov, I.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Anghel, I. M.; Apanasevich, L.; Bai, Y.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Callner, J.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Lacroix, F.; Malek, M.; O'Brien, C.; Silkworth, C.; Strom, D.; Turner, P.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Ozturk, S.; Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Duru, F.; Merlo, J-P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Newsom, C. R.; Norbeck, E.; Onel, Y.; Ozok, F.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Giurgiu, G.; Gritsan, A. V.; Guo, Z. J.; Hu, G.; Maksimovic, P.; Rappoccio, S.; Swartz, M.; Whitbeck, A.] Johns Hopkins Univ, Baltimore, MD USA. [Sphicas, P.; Baringer, P.; Bean, A.; Benelli, G.; Iii, R. P. Kenny; Murray, M.; Noonan, D.; Sanders, S.; Stringer, R.; Tinti, G.; Wood, J. S.; Zhukova, V.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Bolton, T.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Boutemeur, M.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kim, M.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Peterman, A.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.; Twedt, E.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Bauer, G.; Bendavid, J.; Busza, W.; Butz, E.; Cali, I. A.; Chan, M.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Hahn, K. A.; Kim, Y.; Klute, M.; Krajczar, K.; Luckey, P. D.; Ma, T.; Nahn, S.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Rudolph, M.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Sung, K.; Velicanu, D.; Wenger, E. A.; Wolf, R.; Wyslouch, B.; Yang, M.; Yilmaz, Y.; Yoon, A. S.; Zanetti, M.] MIT, Cambridge, MA 02139 USA. [Cooper, S. I.; Dahmes, B.; De Benedetti, A.; Franzoni, G.; Gude, A.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Sasseville, M.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Cremaldi, L. M.; Kroeger, R.; Perera, L.; Rahmat, R.; Sanders, D. A.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Butt, J.; Claes, D. R.; Dominguez, A.; Eads, M.; Keller, J.; Kravchenko, I.; Lazo-Flores, J.; Malbouisson, H.; Malik, S.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Kumar, A.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Nash, D.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Anastassov, A.; Kubik, A.; Mucia, N.; Odell, N.; Ofierzynski, R. A.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Antonelli, L.; Berry, D.; Brinkerhoff, A.; Chan, K. M.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kolb, J.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Morse, D. M.; Pearson, T.; Planer, M.; Ruchti, R.; Slaunwhite, J.; Valls, N.; Wayne, M.; Wolf, M.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Bylsma, B.; Durkin, L. S.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Puigh, D.; Rodenburg, M.; Vuosalo, C.; Williams, G.; Winer, B. L.] Ohio State Univ, Columbus, OH 43210 USA. [Adam, N.; Berry, E.; Elmer, P.; Gerbaudo, D.; Halyo, V.; Hebda, P.; Hegeman, J.; Hunt, A.; Jindal, P.; Pegna, D. Lopes; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Raval, A.; Safdi, B.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Brownson, E.; Lopez, A.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA. [Alagoz, E.; Barnes, V. E.; Benedetti, D.; Lla, G. Bo; Bortoletto, D.; De Mattia, M.; Everett, A.; Hu, Z.; Jones, M.; Koybasi, O.; Kress, M.; Laasanen, A. T.; Leonardo, N.; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Marono, M. Vidal; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Guragain, S.; Parashar, N.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Boulahouache, C.; Ecklund, K. M.; Geurts, F. J. M.; Li, W.; Ley, B. P. Pad; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; Chung, Y. S.; Covarelli, R.; De Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Hard, A.; Miner, D. C.; Vishnevskiy, D.; Zielinski, M.] Univ Rochester, Rochester, NY 14627 USA. [Bhatti, A.; Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Malik, S.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Lath, A.; Panwalkar, S.; Park, M.; Patel, R.; Rekovic, V.; Robles, J.; Rose, K.; Salur, S.; Schnetzer, S.; Seitz, C.; Somalwar, S.; Stone, R.; Thomas, S.] Rutgers State Univ, Piscataway, NJ USA. [Cerizza, G.; Hollingsworth, M.; Spanier, S.; Yang, Z. 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RI Andreev, Vladimir/M-8665-2015; TUVE', Cristina/P-3933-2015; KIM, Tae Jeong/P-7848-2015; Arce, Pedro/L-1268-2014; Flix, Josep/G-5414-2012; Della Ricca, Giuseppe/B-6826-2013; Azarkin, Maxim/N-2578-2015; Dubinin, Mikhail/I-3942-2016; Paganoni, Marco/A-4235-2016; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Seixas, Joao/F-5441-2013; Vilela Pereira, Antonio/L-4142-2016; Stahl, Achim/E-8846-2011; Trocsanyi, Zoltan/A-5598-2009; Konecki, Marcin/G-4164-2015; Hernandez Calama, Jose Maria/H-9127-2015; Bedoya, Cristina/K-8066-2014; My, Salvatore/I-5160-2015; Matorras, Francisco/I-4983-2015; Ragazzi, Stefano/D-2463-2009; Rovelli, Tiziano/K-4432-2015; Dremin, Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Leonidov, Andrey/M-4440-2013; Bargassa, Pedrame/O-2417-2016; Sguazzoni, Giacomo/J-4620-2015; Fassi, Farida/F-3571-2016; Menasce, Dario Livio/A-2168-2016; Sznajder, Andre/L-1621-2016; Haj Ahmad, Wael/E-6738-2016; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; 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Demaria, Natale/0000-0003-0743-9465; Benaglia, Andrea Davide/0000-0003-1124-8450; Covarelli, Roberto/0000-0003-1216-5235; Ciulli, Vitaliano/0000-0003-1947-3396; Bean, Alice/0000-0001-5967-8674; Longo, Egidio/0000-0001-6238-6787; Di Matteo, Leonardo/0000-0001-6698-1735; Baarmand, Marc/0000-0002-9792-8619; Boccali, Tommaso/0000-0002-9930-9299; Menasce, Dario Livio/0000-0002-9918-1686; Sznajder, Andre/0000-0001-6998-1108; Haj Ahmad, Wael/0000-0003-1491-0446; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Gerbaudo, Davide/0000-0002-4463-0878; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Marinho, Franciole/0000-0002-7327-0349; Ferguson, Thomas/0000-0001-5822-3731; Benussi, Luigi/0000-0002-2363-8889; Dahms, Torsten/0000-0003-4274-5476; Grandi, Claudio/0000-0001-5998-3070; Lazzizzera, Ignazio/0000-0001-5092-7531; 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CERN; Chinese Academy of Sciences; Ministry of Science and Technology; National Natural Science Foundation of China; Colombian Funding Agency (COLCIENCIAS); Croatian Ministry of Science, Education and Sport; Research Promotion Foundation; Cyprus; Ministry of Education and Research; European Regional Development Fund, Estonia; Academy of Finland; Finnish Ministry of Education and Culture; Helsinki Institute of Physics; Institut National de Physique Nucleaire et de Physique des Particules / CNRS; Commissariat a l'Energie Atomique et aux Energies Alternatives / CEA, France; Bundesministerium fur Bildung und Forschung; Deutsche Forschungsgemeinschaft; Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; General Secretariat for Research and Technology, Greece; National Scientific Research Foundation; National Office for Research and Technology, Hungary; Department of Atomic Energy; Department of Science and Technology, India; Institute for Studies in Theoretical Physics and Mathematics, Iran; Science Foundation, Ireland; Istituto Nazionale di Fisica Nucleare, Italy; Korean Ministry of Education, Science and Technology; World Class University program of NRF, Korea; Lithuanian Academy of Sciences; CINVESTAV; CONACYT; SEP; UASLP-FAI; Ministry of Science and Innovation, New Zealand; Pakistan Atomic Energy Commission; Ministry of Science and Higher Education; National Science Centre, Poland; Fundacao para a Ciencia e a Tecnologia, Portugal; JINR (Armenia); JINR (Belarus); JINR (Georgia); JINR (Ukraine); JINR (Uzbekistan); Ministry of Education and Science of the Russian Federation; Federal Agency of Atomic Energy of the Russian Federation; Russian Academy of Sciences; Russian Foundation for Basic Research; Ministry of Science and Technological Development of Serbia; Secretaria de Estado de Investigacion; Desarrollo e Innovacion and Programa Consolider-Ingenio, Spain; ETH Board; ETH Zurich; PSI; SNF; UniZH; Canton Zurich; SER; National Science Council, Taipei; Thailand Center of Excellence in Physics; Institute for the Promotion of Teaching Science and Technology; National Electronics and Computer Technology Center; Scientific and Technical Research Council of Turkey; Turkish Atomic Energy Authority; Science and Technology Facilities Council, U.K.; US Department of Energy; US National Science Foundation; Marie-Curie programme; European Research Council (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of Czech Republic; Council of Science and Industrial Research, India; Compagnia di San Paolo (Torino); HOMING PLUS programme of Foundation for Polish Science; European Union; Regional Development Fund; [SF0690030s09] FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centres and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: the Austrian Federal Ministry of Science and Research; the Belgian Fonds de la Recherche Scientifique, and Fonds voor Wetenschappelijk Onderzoek; the Brazilian Funding Agencies (CNPq, CAPES, FAPERJ, and FAPESP); the Bulgarian Ministry of Education, Youth and Science; CERN; the Chinese Academy of Sciences, Ministry of Science and Technology, and National Natural Science Foundation of China; the Colombian Funding Agency (COLCIENCIAS); the Croatian Ministry of Science, Education and Sport; the Research Promotion Foundation, Cyprus; the Ministry of Education and Research, Recurrent financing contract SF0690030s09 and European Regional Development Fund, Estonia; the Academy of Finland, Finnish Ministry of Education and Culture, and Helsinki Institute of Physics; the Institut National de Physique Nucleaire et de Physique des Particules / CNRS, and Commissariat a l'Energie Atomique et aux Energies Alternatives / CEA, France; the Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft, and Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; the General Secretariat for Research and Technology, Greece; the National Scientific Research Foundation, and National Office for Research and Technology, Hungary; the Department of Atomic Energy and the Department of Science and Technology, India; the Institute for Studies in Theoretical Physics and Mathematics, Iran; the Science Foundation, Ireland; the Istituto Nazionale di Fisica Nucleare, Italy; the Korean Ministry of Education, Science and Technology and the World Class University program of NRF, Korea; the Lithuanian Academy of Sciences; the Mexican Funding Agencies (CINVESTAV, CONACYT, SEP, and UASLP-FAI); the Ministry of Science and Innovation, New Zealand; the Pakistan Atomic Energy Commission; the Ministry of Science and Higher Education and the National Science Centre, Poland; the Fundacao para a Ciencia e a Tecnologia, Portugal; JINR (Armenia, Belarus, Georgia, Ukraine, Uzbekistan); the Ministry of Education and Science of the Russian Federation, the Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences, and the Russian Foundation for Basic Research; the Ministry of Science and Technological Development of Serbia; the Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio 2010, Spain; the Swiss Funding Agencies (ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER); the National Science Council, Taipei; the Thailand Center of Excellence in Physics, the Institute for the Promotion of Teaching Science and Technology and National Electronics and Computer Technology Center; the Scientific and Technical Research Council of Turkey, and Turkish Atomic Energy Authority; the Science and Technology Facilities Council, U.K.; the US Department of Energy, and the US National Science Foundation.; Individuals have received support from the Marie-Curie programme and the European Research Council (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of Czech Republic; the Council of Science and Industrial Research, India; the Compagnia di San Paolo (Torino); and the HOMING PLUS programme of Foundation for Polish Science, cofinanced from European Union, Regional Development Fund. NR 55 TC 2 Z9 2 U1 3 U2 100 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JAN PY 2013 IS 1 AR 077 DI 10.1007/JHEP01(2013)077 PG 40 WC Physics, Particles & Fields SC Physics GA 098XU UT WOS:000315583200077 ER PT J AU Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Aguilo, E Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hammer, J Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Pernicka, M Rahbaran, B Rohringer, C Rohringer, H Schofbeck, R Strauss, J Taurok, A Waltenberger, W Walzel, G Widl, E Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Bansal, M Bansal, S Cornelis, T De Wolf, EA Janssen, X Luyckx, S Mucibello, L Ochesanu, S Roland, B Rougny, R Selvaggi, M Staykova, Z Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Suarez, RG Kalogeropoulos, A Maes, M Olbrechts, A Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Clerbaux, B De Lentdecker, G Dero, V Gay, APR Hreus, T Leonard, A Marage, PE Mohammadi, A 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CA CMS Collaboration TI Measurement of the ZZ production cross section and search for anomalous couplings in 2l2l' final states in pp collisions at root s=7 TeV SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering ID Z-GAMMA-GAMMA; PARTON DISTRIBUTIONS; BOSON; LHC; LEP AB A measurement is presented of the ZZ production cross section in the ZZ -> 2l2l' decay mode with l = e, mu and l' = e, mu, tau in proton-proton collisions at root s = 7 TeV with the CMS experiment at the LHC. Results are based on data corresponding to an integrated luminosity of 5.0 fb(-1). The measured cross section sigma(pp -> ZZ) = 6.24(-080)(+0.86) (stat.)(-0.32)(+0.41) (syst.) +/- 0.14 (lumi.) pb is consistent with the standard model predictions. The following limits on ZZZ and ZZ-gamma anomalous trilinear gauge couplings are set at 95% confidence level: -0.011 < f(4)(Z) < 0.012, -0.012 < f(5)(Z) < 0.012, -0.013 < f(4)(gamma) < 0.015, and -0.014 < f(5)(gamma) < 0.014. 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M.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Radi, A.; De Cosa, A.; Dogangun, O.; Iorio, A. O. M.] Univ Naples Federico II, Naples, Italy. [Bacchetta, N.; Bellan, P.; Bisello, D.; Branca, A.; Carlin, R.; Checchia, P.; Dorigo, T.; Dosselli, U.; Gasparini, F.; Gasparini, U.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Lazzizzera, I.; Margoni, M.; Meneguzzo, A. T.; Nespolo, M.; Pazzini, J.; Ronchese, P.; Simonetto, F.; Torassa, E.; Vanini, S.; Zotto, P.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Radi, A.; Bisello, D.; Branca, A.; Carlin, R.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Ronchese, P.; Simonetto, F.; Vanini, S.; Zotto, P.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.; Lazzizzera, I.] Univ Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Torre, P.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Torre, P.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Nappi, A.; Romeo, F.; Saha, A.; Santocchia, A.; Spiezia, A.; Taroni, S.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Radi, A.; Biasini, M.; Fano, L.; Lariccia, P.; Mantovani, G.; Nappi, A.; Romeo, F.; Santocchia, A.; Spiezia, A.; Taroni, S.] Univ Perugia, I-06100 Perugia, Italy. [Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; D'Agnolo, R. T.; Dell'Orso, R.; Fiori, F.; Foa, L.; Giassi, A.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Radi, A.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Azzurri, P.; Broccolo, G.; D'Agnolo, R. T.; Fiori, F.; Foa, L.; Ligabue, F.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Diemoz, M.; Fanelli, C.; Grassi, M.; Longo, E.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Sigamani, M.; Soffi, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Radi, A.; Barone, L.; Del Re, D.; Fanelli, C.; Grassi, M.; Longo, E.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Soffi, L.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Biino, C.; Cartiglia, N.; Costa, M.; Demaria, N.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Pastrone, N.; Pelliccioni, M.; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Radi, A.; Amapane, N.; Argiro, S.; Costa, M.; Migliore, E.; Monaco, V.; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; Marone, M.; Montanino, D.; Penzo, A.; Schizzi, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Radi, A.; Candelise, V.; Della Ricca, G.; Marone, M.; Montanino, D.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Heo, S. G.; Kim, T. Y.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Chang, S.; Kim, D. H.; Kim, G. N.; Kong, D. J.; Ro, S. R.; Son, D. C.; Son, T.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, J. Y.; Kim, Zero J.; Song, S.] Chonnam Natl Univ, Inst Univ & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, T. J.; Lee, K. S.; Moon, D. H.; Park, S. K.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Cho, Y.; Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. S.; Kwon, E.; Lee, B.; Lee, J.; Lee, S.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Bilinskas, M. J.; Grigelionis, I.; Janulis, M.; Juodagalvis, A.] Vilnius State Univ, Vilnius, Lithuania. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Lopez-Fernandez, R.; Magana Villalba, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.; Reyes-Santos, M. A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Bell, A. J.; Butler, P. H.; Doesburg, R.; Reucroft, S.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Asghar, M. I.; Butt, J.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Boimska, B.; Frueboes, T.; Gokieli, R.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Almeida, N.; Bargassa, P.; David, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Belotelov, I.; Bunin, P.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Kozlov, G.; Lanev, A.; Malakhov, A.; Moisenz, P.; Palichik, V.; Perelygin, V.; Savina, M.; Shmatov, S.; Smirnov, V.; Volodko, A.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Evstyukhin, S.; Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Matveev, V.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Erofeeva, M.; Gavrilov, V.; Kossov, M.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Stolin, V.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Markina, A.; Obraztsov, S.; Perfilov, M.; Petrushanko, S.; Popov, A.; Sarycheva, L.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Grishin, V.; Kachanov, V.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Alcaraz Maestre, J.; Arce, P.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De la Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Santaolalla, L. Romero J.; Soares, M. S.; Willmott, C.] Ctr Invest Eneret Medioambientales & Tecnol CIEMA, Madrid, Spain. [Albajar, C.; Codispoti, G.; de Troconiz, J. F.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.; Piedra Gomez, J.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Chuang, S. H.; Duarte Campderros, J.; Felcini, M.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Graziano, A.; Jorda, C.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benitez, J. 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Palencia; Perez, E.; Perrozzi, L.; Petrilli, A.; Pfeiffer, A.; Pierini, M.; Pimia, M.; Piparo, D.; Polese, G.; Quertenmont, L.; Racz, A.; Reece, W.; Antunes, J. Rodrigues; Rolandi, G.; Rovelli, C.; Rovere, M.; Sakulin, H.; Santanastasio, F.; Schaefer, C.; Schwick, C.; Segoni, I.; Sekmen, S.; Sharma, A.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Tsirou, A.; Veres, G. I.; Vlimant, J. R.; Woehri, H. K.; Worm, S. D.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Gabathuler, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Meier, F.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Baeni, L.; Bortignon, P.; Buchmann, M. A.; Casal, B.; Chanon, N.; Deisher, A.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eugster, J.; Freudenreich, K.; Grab, C.; Hits, D.; Lecomte, P.; Lustermann, W.; Marini, A. C.; del Arbol, P. Martinez Ruiz; Mohr, N.; Moortgat, F.; Naegeli, C.; Nef, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pape, L.; Pauss, F.; Peruzzi, M.; Ronga, F. J.; Rossini, M.; Sala, L.; Sanchez, A. K.; Starodumov, A.; Stieger, B.; Takahashi, M.; Tauschert, L.; Thea, A.; Theofilatos, K.; Treille, D.; Urscheler, C.; Wallny, R.; Weber, H. A.; Wehrli, L.] ETH, Inst Particle Phys, Zurich, Switzerland. [Amsler, C.; Chiochia, V.; De Visscher, S.; Favaro, C.; Rikova, M. Ivova; Mejias, B. Millan; Otiougova, P.; Robmann, P.; Snoek, H.; Tupputi, S.; Verzetti, M.] Univ Zurich, Zurich, Switzerland. [Chang, Y. H.; Chen, K. H.; Kuo, C. M.; Li, S. W.; Lin, W.; Lu, Y. J.; Mekterovic, D.; Singh, A. P.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Dietz, C.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wan, X.; Wang, M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Srimanobhas, N.] Chulalongkorn Univ, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Karaman, T.; Karapinar, G.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tai, B.; Topakli, H.; Vergili, L. N.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Yildirim, E.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey. [Cankocak, K.; Levchuk, L.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Kreczko, L.; Metson, S.; Newbold, D. M.; Nirunpong, K.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Basso, L.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Jackson, J.; Kennedy, B. W.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Womersley, W. J.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Bainbridge, R.; Ball, G.; Beuselinck, R.; Buchmuller, O.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Papageorgiou, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Ryan, M. J.; Seez, C.; Sharp, P.; Sparrow, A.; Stoye, M.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.; Whyntie, T.] Univ London Imperial Coll Sci Technol & Med, London, England. [Chadwick, M.; Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Hatakeyama, K.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; St John, J.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Bhattacharya, S.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Nguyen, D.; Segala, M.; Sinthuprasith, T.; Speer, T.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De la Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Dolen, J.; Erbacher, R.; Gardner, M.; Houtz, R.; Ko, W.; Kopecky, A.; Lander, R.; Mall, O.; Miceli, T.; Pellett, D.; Ricci-Tam, F.; Rutherford, B.; Searle, M.; Smith, J.; Squires, M.; Tripathi, M.; Sierra, R. Vasquez; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Andreev, V.; Cline, D.; Cousins, R.; Duris, J.; Erhan, S.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Plager, C.; Rakness, G.; Schlein, P.; Traczyk, P.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Babb, J.; Clare, R.; Dinardo, M. E.; Ellison, J.; Gary, J. 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High Energy Phys. PD JAN PY 2013 IS 1 AR 063 DI 10.1007/JHEP01(2013)063 PG 29 WC Physics, Particles & Fields SC Physics GA 098XU UT WOS:000315583200063 ER PT J AU Chen, Y Tran, N Vega-Morales, R AF Chen, Yi Nhan Tran Vega-Morales, Roberto TI Srutinizing the Higgs signal and background in the 2e2 mu golden channel SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Higgs Physics; Standard Model ID Z-BOSON PAIRS; LEPTONIC SIGNALS; HADRON COLLIDERS; LHC; DECAYS; MASS; SPIN AB Kinematic distributions in the decays of the newly discovered resonance to four leptons are a powerful probe of the tensor structure of its couplings to electroweak gauge bosons. We present analytic calculations for both signal and background of the fully differential cross section for the 'Golden Channel' e(+)e(-)mu(+)mu(-) final state. We include all interference effects between intermediate gauge bosons and allow them to be on- or off-shell. For the signal we compute the fully differential decay width for general scalar couplings to ZZ, gamma gamma, and Z gamma. For the background we compute the leading order fully differential cross section for q (q) over bar annihilation into Z and gamma gauge bosons, including the contribution from the resonant Z -> 2e2 mu process. We also present singly and doubly differential projections and study the interference effects on the differential spectra. These expressions can be used in a variety of ways to uncover the nature of the newly discovered resonance or any new scalars decaying to neutral gauge bosons which might be discovered in the future. C1 [Chen, Yi] CALTECH, Dept Phys, Pasadena, CA 91125 USA. [Nhan Tran; Vega-Morales, Roberto] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Vega-Morales, Roberto] Northwestern Univ, Dept Phys & Astron, Evanston, IL 60208 USA. RP Vega-Morales, R (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. EM yichen@caltech.edu; ntran@fnal.gov; robertovegamorales2010@u.northwestern.edu FU Fermilab Graduate Student Fellowship program; Weston Havens Foundation; DOE [DE-FG02-92-ER-40701]; Fermi Research Alliance, LLC [De-AC02-07CH11359]; United States Department of Energy FX We thank Joe Lykken, Ian Low, Andrei Gritsan, and Maria Spiropulu for helpful discussions. R. V. M. is especially grateful to Kunal Kumar for help with validation and numerous discussions. N.T. is grateful to Andrew Whitbeck and Ian Anderson for consultation. R. V. M. is supported by the Fermilab Graduate Student Fellowship program. Y.C. is supported by the Weston Havens Foundation and DOE grant DE-FG02-92-ER-40701. This research is also partially supported by Fermi Research Alliance, LLC under Contract No. De-AC02-07CH11359 with the United States Department of Energy. NR 38 TC 15 Z9 15 U1 0 U2 3 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JAN PY 2013 IS 1 AR 182 DI 10.1007/JHEP01(2013)182 PG 30 WC Physics, Particles & Fields SC Physics GA 098XY UT WOS:000315583600101 ER PT J AU Hall, LJ Nomura, Y Shirai, S AF Hall, Lawrence J. Nomura, Yasunori Shirai, Satoshi TI Spread Supersymmetry with (W)over-tilde LSP: gluino and dark matter signals SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Supersymmetry Phenomenology ID MU-PROBLEM; COSMOLOGICAL CONSTANT; SPLIT SUPERSYMMETRY; ANOMALY MEDIATION; NATURAL SOLUTION; STANDARD MODEL; WINO LSP; SUPERGRAVITY; BREAKING; LHC AB The discovery of a Higgs boson near 125GeV, together with the absence of LHC signals for supersymmetry or direct detection signals of dark matter, motivate further study of a particular theory of split supersymmetry. In arguably the theoretically simplest implementation of split, the superpartner spectrum is spread over several decades. The squarks and sleptons are heavier than the gravitino and Higgsinos by a factor M-Pl/M-*, where M-* is the mediation scale of supersymmetry breaking and is high, between unified and Planck scales. On the other hand the gaugino masses are 1-loop smaller than the gravitino and Higgsino masses, arising from both anomaly mediation and a Higgsino loop. Wino dark matter arises from three sources: gravitino production by scattering at high temperatures, gravitino production from squark decays, and thermal freeze-out. For reheating temperatures larger than the squark mass, these conspire to require that the squarks are lighter than about 10(4) TeV, while collider limits on gaugino masses require squarks to be heavier than about 100 TeV. Whether winos constitute all or just a fraction of the dark matter, a large fraction of the allowed parameter space has the gluino within reach of the LHC with 0.1 mm < c tau(<(g)over tilde>) < 10 cm, leading to displaced vertices. In addition, events with cascades via <(W)over tilde>(+/-) lead to disappearing charged tracks with c tau((W) over tilde+/-) similar to 10 cm. The squarks and sleptons are predicted to be just heavy enough to solve the supersymmetric flavor and CP problems. Thus gluino decay modes may typically violate flavor and involve heavy quarks: [(t) over bar (t, c, u) + (b) over bar (b, s, d)](W) over tilde (0) and [(t) over bar (b, s, d) + ((t) over bar, (c) over bar, (u) over bar )b](W) over tilde (+/-). The electron electric dipole moment is expected to be of order 10(-29) e cm, two orders of magnitude below the current limit. The AMS-02 search for cosmic ray antiprotons will probe an interesting region of parameter space. C1 [Hall, Lawrence J.; Nomura, Yasunori; Shirai, Satoshi] Univ Calif Berkeley, Dept Phys, Berkeley Ctr Theoret Phys, Berkeley, CA 94720 USA. [Hall, Lawrence J.; Nomura, Yasunori; Shirai, Satoshi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Theoret Phys Grp, Berkeley, CA 94720 USA. [Nomura, Yasunori] MIT, Ctr Theoret Phys, Nucl Sci Lab, Cambridge, MA 02139 USA. [Nomura, Yasunori] MIT, Dept Phys, Cambridge, MA 02139 USA. RP Hall, LJ (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley Ctr Theoret Phys, Berkeley, CA 94720 USA. EM ljhall@lbl.gov; ynomura@berkeley.edu; shirai@berkeley.edu FU Office of Science, Office of High Energy and Nuclear Physics, of the U.S. Department of Energy [DE-FG02-05ER41360, DE-AC02-05CH11231]; National Science Foundation [PHY-0855653, PHY-1002399, PHY-1066293]; EU ITN [UNILHC 237920]; Simons Foundation [230224] FX S.S. thanks N. Nagata for valuable discussions. This work was supported in part by the Director, Office of Science, Office of High Energy and Nuclear Physics, of the U.S. Department of Energy under Contracts DE-FG02-05ER41360 and DE-AC02-05CH11231, by the National Science Foundation under grants PHY-0855653 and PHY-1002399, by the EU ITN grant UNILHC 237920 (Unification in the LHC era), and by the Simons Foundation grant 230224. L.J.H. and Y.N. acknowledge the hospitality of the Aspen Center for Physics, which is supported by the National Science Foundation Grant No. PHY-1066293. NR 102 TC 52 Z9 52 U1 0 U2 2 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JAN PY 2013 IS 1 AR 036 DI 10.1007/JHEP01(2013)036 PG 32 WC Physics, Particles & Fields SC Physics GA 098XU UT WOS:000315583200036 ER PT J AU Schweitzer, P Strikman, M Weiss, C AF Schweitzer, P. Strikman, M. Weiss, C. TI Intrinsic transverse momentum and parton correlations from dynamical chiral symmetry breaking SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Deep Inelastic Scattering; Phenomenological Models; Parton Model; QCD ID ANTIQUARK FLAVOR ASYMMETRY; QUARK-GLUON CONDENSATE; ROOT S=1.8 TEV; DRELL-YAN PAIR; N-C LIMIT; QUANTUM CHROMODYNAMICS; (P)OVER-BAR-P COLLISIONS; MULTIPARTON INTERACTIONS; FRAGMENTATION FUNCTIONS; NUCLEON CORRELATIONS AB The dynamical breaking of chiral symmetry in QCD is caused by nonperturbative interactions on a distance scale rho similar to 0.3 fm, much smaller than the typical hadronic size R similar to 1 fm. These short-distance interactions influence the intrinsic transverse momentum distributions of partons and their correlations at a low normalization point. We study this phenomenon in an effective description of the low-energy dynamics in terms of chiral constituent quark degrees of freedom, which refers to the large-N-c limit of QCD. The nucleon is obtained as a system of constituent quarks and antiquarks moving in a self-consistent classical chiral field (relativistic mean-field approximation, or chiral quark-soliton model). The calculated transverse,. momentum distributions of constituent quarks and antiquarks are matched with QCD quarks, antiquarks and gluons at the chiral symmetry-breaking scale rho(-2). We find that the transverse momentum distribution of valence quarks is localized at p(T)(2) similar to R-2 and roughly of Gaussian shape. The distribution of unpolarized sea quarks exhibits a would-be power-like tail similar to 1/p(T)(2) extending up to the chiral symmetry-breaking scale. Similar behavior is observed in the flavor-nonsinglet polarized sea. The high-momentum tails are the result of short-range correlations between sea quarks in the nucleon's light-cone wave function, which are analogous to short-range NN correlations in nuclei. We show that the nucleon's light-cone wave function contains correlated pairs of transverse size rho << R with scalar-isoscalar (Sigma) and pseudoscalar-isovector (Pi) quantum numbers, whose internal wave functions have a distinctive spin structure and become identical at p(T)(2) similar to rho(-2) (restoration of chiral symmetry). These features are model-independent and represent an effect of dynamical chiral symmetry breaking on the nucleon's partonic structure. Our results have numerous implications for the transverse momentum distributions of particles produced in hard scattering processes. Under certain conditions the nonperturbative part on correlations predicted here could be observed in particle correlations between the current and target fragmentation regions of deep-inelastic scattering. C1 [Schweitzer, P.] Univ Connecticut, Dept Phys, Storrs, CT 06269 USA. [Strikman, M.] Penn State Univ, Dept Phys, University Pk, PA 16802 USA. [Weiss, C.] Jefferson Lab, Ctr Theory, Newport News, VA 23606 USA. RP Schweitzer, P (reprint author), Univ Connecticut, Dept Phys, Storrs, CT 06269 USA. EM peter.schweitzer@phys.uconn.edu; strikman@phys.psu.edu; weiss@jlab.org FU U.S. DOE [DE-FGO2-93ER40771, DE-AC05-06OR23177] FX M. S. acknowledges the hospitality of Jefferson Lab during the work on this study. This work is supported by the U.S. DOE under Grant No. DE-FGO2-93ER40771. Notice: authored by Jefferson Science Associates, LLC under U.S. DOE Contract No. DE-AC05-06OR23177. The U.S. Government retains a non-exclusive, paid-up, irrevocable, worldwide license to publish or reproduce this manuscript for U.S. Government purposes. NR 122 TC 20 Z9 20 U1 0 U2 1 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JAN PY 2013 IS 1 AR 163 DI 10.1007/JHEP01(2013)163 PG 90 WC Physics, Particles & Fields SC Physics GA 098XY UT WOS:000315583600082 ER PT J AU Senatore, L Zaldarriaga, M AF Senatore, Leonardo Zaldarriaga, Matias TI On loops in inflation II: IR effects in single clock inflation SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Cosmology of Theories beyond the SM; Gauge Symmetry; Space-Time Symmetries; Renormalization Regularization and Renormalons AB In single clock models of inflation the coupling between modes of very different scales does not have any significant dynamical effect during inflation. It leads to interesting projection effects. Larger and smaller modes change the relation between the scale a mode of interest will appear in the post-inflationary universe and will also change the time of horizon crossing of that mode. We argue that there are no infrared projection effects in physical questions, that there are no effects from modes of longer wavelength than the one of interest at the time of reheating. These potential effects cancel when computing fluctuations as a function of physically measurable scales. Modes on scales smaller than the one of interest change the mapping between horizon crossing time and scale. The correction to the mapping computed in the absence of fluctuations is enhanced by a factor N-e, the number of e-folds of inflation between horizon crossing and reheating. The new mapping is stochastic in nature but its variance is not enhanced by N-e. C1 [Senatore, Leonardo] Stanford Univ, Stanford Inst Theoret Phys, Stanford, CA 94306 USA. [Senatore, Leonardo] Stanford Univ, Kavli Inst Particle Astrophys & Cosmol, Menlo Pk, CA 94025 USA. [Senatore, Leonardo] SLAC, Menlo Pk, CA 94025 USA. [Zaldarriaga, Matias] Inst Adv Study, Sch Nat Sci, Princeton, NJ 08540 USA. RP Senatore, L (reprint author), Stanford Univ, Stanford Inst Theoret Phys, 382 Via Pueblo Mall, Stanford, CA 94306 USA. EM senatore@stanford.edu; matiasz@ias.edu FU National Science Foundation [PHY-1068380, PHY- 0855425, AST-0907969]; David and Lucile Packard Foundation; John D. and Catherine T. MacArthur Foundation FX We thank Nima Arkani-Hamed, Steve Giddings, Richard Holman, Shamit Kachru, Juan Maldacena, Steve Shenker, Eva Silverstein and Lenny Susskind for interesting conversations. L.S. is supported by the National Science Foundation under PHY-1068380. M.Z. is supported by the National Science Foundation under PHY- 0855425 and AST-0907969 and by the David and Lucile Packard Foundation and the John D. and Catherine T. MacArthur Foundation. NR 27 TC 20 Z9 20 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JAN PY 2013 IS 1 AR 109 DI 10.1007/JHEP01(2013)109 PG 15 WC Physics, Particles & Fields SC Physics GA 098XY UT WOS:000315583600028 ER PT J AU Liu, B Abouimrane, A Brown, DE Zhang, XF Ren, Y Fang, ZZ Amine, K AF Liu, Bo Abouimrane, Ali Brown, Dennis E. Zhang, Xiaofeng Ren, Yang Fang, Zhigang Zak Amine, Khalil TI Mechanically alloyed composite anode materials based on SiO-SnxFeyCz for Li-ion batteries SO JOURNAL OF MATERIALS CHEMISTRY A LA English DT Article ID X-RAY-DIFFRACTION; TIN-COBALT-CARBON; IN-SITU; NEGATIVE ELECTRODES; SN-FE(-C) POWDERS; ELECTROCHEMICAL REACTION; LITHIUM; COMBINATORIAL; SYSTEM AB A new family of composite materials as anodes for lithium-ion batteries, SiO-SnxFeyCz (x : y : z molar ratio), was synthesized by mechanical alloying. SiO is preferable because of its high capacity and the Sn-Fe-C alloys could be used as a buffer material to extend the cycle life of cells. Rather than expensive and toxic cobalt, we selected cheap and environmentally benign iron instead. The aim of this work is to find the optimal point by tuning the composition of Sn-Fe-C in the hope of obtaining better electrochemical performance. Different combinations were studied by high-energy X-ray diffraction and electrochemical methods. The results indicated that carbon can improve the cycle life, the amount of iron affects phase formation greatly, and the FeSn2 phase should be avoided because of its detrimental effect on cycle life. The 50 wt% SiO-50 wt% Sn30Fe30C40 composition was studied using the pair distribution function and Mossbauer spectroscopy. This material exhibits high specific capacity (900 mA h g(-1) at C/6 rate) with good cycle life and rate capability. These results indicate that SiO-SnxFeyCz are promising candidate anode materials for commercial rechargeable lithium batteries. C1 [Liu, Bo; Abouimrane, Ali; Zhang, Xiaofeng; Amine, Khalil] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Liu, Bo; Fang, Zhigang Zak] Univ Utah, Dept Met Engn, Salt Lake City, UT 84112 USA. [Brown, Dennis E.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Ren, Yang] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. RP Liu, B (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM Abouimrane@anl.gov; zak.fang@utah.edu; Amine@anl.gov RI Amine, Khalil/K-9344-2013 FU Applied Battery Research for Transportation program (Department of Energy); Institute of NanoScience, Engineering, and Technology (INSET) of Northern Illinois University; U.S. Department of Energy Office of Science laboratory [DE-AC02-06CH11357] FX Funding from the Applied Battery Research for Transportation program (Department of Energy) is gratefully acknowledged. This work was also supported by the Institute of NanoScience, Engineering, and Technology (INSET) of Northern Illinois University. It has benefited from the use of the beamline 11-ID-C at the Advanced Photon Source. The submitted manuscript has been created by UChicago Argonne, LLC, Operator of Argonne National Laboratory ("Argonne"). Argonne, a U.S. Department of Energy Office of Science laboratory, is operated under Contract no. DE-AC02-06CH11357. NR 22 TC 10 Z9 10 U1 1 U2 48 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2050-7488 J9 J MATER CHEM A JI J. Mater. Chem. A PY 2013 VL 1 IS 13 BP 4376 EP 4382 DI 10.1039/c3ta00101f PG 7 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Energy & Fuels; Materials Science GA 100RS UT WOS:000315720000033 ER PT J AU Fang, F Iyyamperumal, E Chi, MF Keskar, G Majewska, M Ren, F Liu, CC Haller, GL Pfefferle, LD AF Fang, Fang Iyyamperumal, Eswaramoorthi Chi, MiaoFang Keskar, Gayatri Majewska, Magdalena Ren, Fang Liu, Changchang Haller, Gary L. Pfefferle, Lisa D. TI Templated one-step catalytic fabrication of uniform diameter MgxBy nanostructures SO JOURNAL OF MATERIALS CHEMISTRY C LA English DT Article ID WALLED CARBON NANOTUBES; SUPERCONDUCTING MGB2 NANOWIRES; RAY-ABSORPTION-SPECTROSCOPY; CHEMICAL-VAPOR-DEPOSITION; THIN-FILMS; ELECTRONIC-STRUCTURE; BORON; DIBORANE; PYROLYSIS; B2H6 AB Direct fabrication of MgxBy nanostructures is achieved by employing Ni-Mg incorporated MCM-41 in the Hybrid Physical-Chemical Vapor Deposition (HPCVD) reaction. Different reaction conditions are tested to optimize the fabrication process. TEM analysis shows the fabrication of MgxBy nanostructures starting at a reaction temperature of 600 degrees C, and the yield of the nanostructures increases with the reaction temperature. The as-synthesized MgxBy nanostructures have the diameters in the range of 3-5 nm, which do not increase with the reaction temperature. EELS analysis of the template removed nanostructures confirms the existence of B and Mg with minimal contamination of Si and O. NEXAFS and Raman spectroscopy analyses suggested a concentric layered structure for our as-synthesized MgxBy nanotube/nanowire, which is in good agreement with the theoretical calculations. Ni K-edge XAS indicates that the formation of MgNi alloy particles is important for the Vapor-Liquid-Solid (VLS) growth of MgxBy nanostructures with fine diameters, and the presence of Mg vapor not just Mg in the catalyst is crucial for the formation of Ni-Mg clusters. Physical templating by MCM-41 might also help to confine the diameter of the nanostructures. DC magnetization measurements indicate possible superconductive behaviors in the as-synthesized sample. C1 [Fang, Fang; Iyyamperumal, Eswaramoorthi; Keskar, Gayatri; Majewska, Magdalena; Ren, Fang; Liu, Changchang; Haller, Gary L.; Pfefferle, Lisa D.] Yale Univ, Dept Chem Engn, New Haven, CT 06520 USA. [Chi, MiaoFang] Oak Ridge Natl Lab, Div Mat Sci, Oak Ridge, TN 37830 USA. RP Fang, F (reprint author), Yale Univ, Dept Chem Engn, 9 Hillhouse Ave, New Haven, CT 06520 USA. EM chim@ornl.gov; lisa.pfefferle@yale.edu RI Chi, Miaofang/Q-2489-2015 OI Chi, Miaofang/0000-0003-0764-1567 FU U.S. Department of Energy, Office of Basic Energy Science [DE-FG02-06ER46322]; MRSEC [DMR 0520495] FX The authors gratefully acknowledge the financial support from the U.S. Department of Energy, Office of Basic Energy Science Grant no. DE-FG02-06ER46322. The authors also acknowledge the use of National Synchrotron Light Source (Beamline U7A, X18B and X23A2) at Brookhaven National Laboratory with the generous help from Dr Daniel Fischer, Dr Cherno Jaye, Dr Nebojsa Marinkovic, and Dr Bruce Ravel; the use of STEM/EELS at Oak Ridge National Laboratory through ORNL SHaRE program, and Yale facilities supported by MRSEC DMR 0520495 (CRISP) for the use of DC SQUID for magnetic measurements. NR 47 TC 1 Z9 1 U1 0 U2 31 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2050-7526 EI 2050-7534 J9 J MATER CHEM C JI J. Mater. Chem. C PY 2013 VL 1 IS 14 BP 2568 EP 2576 DI 10.1039/c3tc00697b PG 9 WC Materials Science, Multidisciplinary; Physics, Applied SC Materials Science; Physics GA 106DD UT WOS:000316121100010 ER PT J AU Adams, BW Buth, C Cavaletto, SM Evers, J Harman, Z Keitel, CH Palffy, A Picon, A Rohlsberger, R Rostovtsev, Y Tamasaku, K AF Adams, Bernhard W. Buth, Christian Cavaletto, Stefano M. Evers, Joerg Harman, Zoltan Keitel, Christoph H. Palffy, Adriana Picon, Antonio Roehlsberger, Ralf Rostovtsev, Yuri Tamasaku, Kenji TI X-ray quantum optics SO JOURNAL OF MODERN OPTICS LA English DT Review DE X-ray quantum optics; parametric down conversion; single-photon superradiance; collective Lamb shift; coherent control; EIT; resonance fluorescence ID ELECTROMAGNETICALLY INDUCED TRANSPARENCY; HIGH-HARMONIC-GENERATION; COHERENT POPULATION TRANSFER; PARAMETRIC DOWN-CONVERSION; COOPERATIVE LAMB SHIFT; DRIVEN 3-LEVEL SYSTEM; FREE-ELECTRON LASER; RESONANCE FLUORESCENCE; SPONTANEOUS EMISSION; EXTREME-ULTRAVIOLET AB Quantum optics with X-rays has long been a somewhat exotic activity, but it is now rapidly becoming relevant as precision x-ray optics and novel X-ray light sources, and high-intensity lasers are becoming available. This article gives an overview of the current state of the field and an outlook to future prospects. C1 [Adams, Bernhard W.; Buth, Christian; Picon, Antonio] Argonne Natl Lab, Argonne, IL 60439 USA. [Cavaletto, Stefano M.; Evers, Joerg; Harman, Zoltan; Keitel, Christoph H.; Palffy, Adriana] Max Planck Inst Nucl Phys, D-69117 Heidelberg, Germany. [Harman, Zoltan] ExtreMe Matter Inst EMMI, D-64291 Darmstadt, Germany. [Roehlsberger, Ralf] Deutsches Elektronen Synchrotron DESY, D-22607 Hamburg, Germany. [Rostovtsev, Yuri] Univ N Texas, Dept Phys, Denton, TX 76203 USA. [Tamasaku, Kenji] RIKEN SPring 8 Ctr, Sayo, Hyogo 6795148, Japan. RP Adams, BW (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. EM adams@aps.anl.gov RI Picon Alvarez, Antonio/I-7268-2012; Evers, Jorg/A-5077-2009; Rohlsberger, Ralf/J-4173-2013; Palffy, Adriana /C-7330-2014; Tamasaku, Kenji/N-7907-2015; Buth, Christian/A-2834-2017 OI Picon Alvarez, Antonio/0000-0002-6142-3440; Evers, Jorg/0000-0001-7864-6029; Rohlsberger, Ralf/0000-0001-6005-5183; Buth, Christian/0000-0002-5866-3443 FU U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-06CH11357]; Alliance Program of the Helmholtz Association [HA216/EMMI]; UNT Research Initiation Grant; summer fellowship UNT program FX This work was supported by the U.S. Department of Energy, Office of Basic Energy Sciences under Contract No. DE-AC02-06CH11357, and by the Alliance Program of the Helmholtz Association (HA216/EMMI). Y.R. gratefully acknowledges the support from the UNT Research Initiation Grant and the summer fellowship UNT program. NR 222 TC 44 Z9 44 U1 7 U2 72 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND SN 0950-0340 EI 1362-3044 J9 J MOD OPTIC JI J. Mod. Opt. PD JAN 1 PY 2013 VL 60 IS 1 SI SI BP 2 EP 21 DI 10.1080/09500340.2012.752113 PG 20 WC Optics SC Optics GA 101JD UT WOS:000315770400002 ER PT J AU Boreyko, JB Mruetusatorn, P Retterer, ST Collier, CP AF Boreyko, Jonathan B. Mruetusatorn, Prachya Retterer, Scott T. Collier, C. Patrick TI Aqueous two-phase microdroplets with reversible phase transitions SO LAB ON A CHIP LA English DT Article ID MICROFLUIDIC DEVICE; INTERFACIAL-TENSION; POLYETHYLENE-GLYCOL; GIANT VESICLES; MICROCOMPARTMENTATION; SEPARATION; SYSTEMS; CELLS; FLOW; MICROCHANNELS AB Aqueous two-phase systems contained within microdroplets enable a bottom-up approach to mimicking the dynamic microcompartmentation of biomaterial that naturally occurs within the cytoplasm of cells. Here, we demonstrate the generation of femtolitre aqueous two-phase droplets within a microfluidic oil channel. Gated pressure pulses were used to generate individual, stationary two-phase microdroplets with a well-defined time zero for carrying out controlled and sequential phase transformations over time. Reversible phase transitions between single-phase, two-phase, and core-shell microbead states were obtained via evaporation-induced dehydration and water rehydration. In contrast to other microfluidic aqueous two-phase droplets, which require continuous flows and high-frequency droplet formation, our system enables the controlled isolation and reversible transformation of a single microdroplet and is expected to be useful for future studies in dynamic microcompartmentation and affinity partitioning. C1 [Boreyko, Jonathan B.; Retterer, Scott T.; Collier, C. Patrick] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Mruetusatorn, Prachya] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Retterer, Scott T.] Oak Ridge Natl Lab, Biosci Div, Biol & Nanoscale Syst Grp, Oak Ridge, TN 37831 USA. RP Collier, CP (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM colliercp@ornl.gov RI Retterer, Scott/A-5256-2011 OI Retterer, Scott/0000-0001-8534-1979 FU Scientific User Facilities Division, Office of Basic Energy Sciences, U. S. Department of Energy FX This research was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U. S. Department of Energy. NR 49 TC 10 Z9 10 U1 4 U2 91 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1473-0197 J9 LAB CHIP JI Lab Chip PY 2013 VL 13 IS 7 BP 1295 EP 1301 DI 10.1039/c3lc41122b PG 7 WC Biochemical Research Methods; Chemistry, Multidisciplinary; Nanoscience & Nanotechnology SC Biochemistry & Molecular Biology; Chemistry; Science & Technology - Other Topics GA 100HI UT WOS:000315688500011 PM 23381219 ER PT J AU Hatch, AC Patel, A Beer, NR Lee, AP AF Hatch, Andrew C. Patel, Apurva Beer, N. Reginald Lee, Abraham P. TI Passive droplet sorting using viscoelastic flow focusing SO LAB ON A CHIP LA English DT Article ID REYNOLDS-NUMBER MOTION; PLANE POISEUILLE FLOW; NON-NEWTONIAN FLUIDS; SHEAR-FLOW; SOFT LITHOGRAPHY; 2ND-ORDER FLUID; DEFORMABLE DROP; MIGRATION; MICROCHANNEL; SEPARATION AB We present a study of passive hydrodynamic droplet sorting in microfluidic channels based on intrinsic viscoelastic fluid properties. Sorting is achieved by tuning the droplets' intrinsic viscous and viscoelastic properties relative to the continuous oil phase to achieve a positive or negative lateral migration toward high or low shear gradients in the channel. In the presence of weakly viscoelastic fluid behavior, droplets with a viscosity ratio, kappa, between 0.5-10 were found to migrate toward a high shear gradient near the channel walls. For all other kappa-values, or Newtonian fluids, droplets would migrate toward a low shear gradient at the channel centerline. It was also found that for strongly viscoelastic fluids with low interfacial tension, droplets would migrate toward the edge even with kappa-values lower than 0.5. The resulting bidirectional lateral droplet migration between different droplets allows size-independent sorting. Still, their sorting efficiencies are dependent on droplet size, intrinsic fluid elasticity, viscosity, droplet deformability, and overall fluid shear rates. Based on these findings, we demonstrate >200 Hz passive droplet sorting frequencies and achieve >100 fold enrichment factors without the need to actively sense and/or control active mechanisms. Using a low viscosity oil phase of 6.25 cPs, we demonstrate sorting discrimination of 1 cPs and 5 cPs aqueous droplets with kappa-values of 0.2 and 0.8 respectively. C1 [Hatch, Andrew C.; Patel, Apurva; Lee, Abraham P.] Univ Calif Irvine, Irvine, CA 92697 USA. [Beer, N. Reginald] Lawrence Livermore Natl Lab, Ctr Micro & Nanotechnol, Livermore, CA 94550 USA. RP Lee, AP (reprint author), Univ Calif Irvine, Irvine, CA 92697 USA. EM ahatch@uci.edu; aplee@uci.edu FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Defense Advanced Research Projects Agency (DARPA) N/MEMS S&T Fundamentals Program [N66001-1-4003] FX The authors thank Dr Jeffrey S. Fisher and Dr Arezoo M. Ardekani for technical contributions to the work. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. This work was also supported in part by the Defense Advanced Research Projects Agency (DARPA) N/MEMS S&T Fundamentals Program under grant no. N66001-1-4003 issued by the Space and Naval Warfare Systems Center Pacific (SPAWAR) to the Micro/nano Fluidics Fundamentals Focus (MF3) Center. NR 55 TC 8 Z9 9 U1 5 U2 56 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1473-0197 J9 LAB CHIP JI Lab Chip PY 2013 VL 13 IS 7 BP 1308 EP 1315 DI 10.1039/c2lc41160a PG 8 WC Biochemical Research Methods; Chemistry, Multidisciplinary; Nanoscience & Nanotechnology SC Biochemistry & Molecular Biology; Chemistry; Science & Technology - Other Topics GA 100HI UT WOS:000315688500013 PM 23380996 ER PT J AU Deng, L Gregory, A Yilmaz, S Poulos, BT Hugenholtz, P Sullivan, MB AF Deng, Li Gregory, Ann Yilmaz, Suzan Poulos, Bonnie T. Hugenholtz, Philip Sullivan, Matthew B. TI Contrasting Life Strategies of Viruses That Infect Photo- and Heterotrophic Bacteria, as Revealed by Viral Tagging (vol 3, e00373, 2012) SO MBIO LA English DT Correction C1 [Deng, Li; Gregory, Ann; Poulos, Bonnie T.; Sullivan, Matthew B.] Univ Arizona, Ecol & Evolutionary Biol Dept, Tucson, AZ USA. [Yilmaz, Suzan; Hugenholtz, Philip] DOE Joint Genome Inst, Microbial Ecol Program, Walnut Creek, CA USA. [Hugenholtz, Philip] Univ Queensland, Australian Ctr Ecogen, Sch Chem & Mol Biosci, St Lucia, Qld, Australia. [Hugenholtz, Philip] Univ Queensland, Inst Mol Biosci, St Lucia, Qld, Australia. RP Deng, L (reprint author), Munchen German Res Ctr Environm Hlth, Helmholtz Zentrum, Inst Groundwater Ecol, Neuherberg, Germany. RI Hugenholtz, Philip/G-9608-2011 NR 1 TC 1 Z9 1 U1 2 U2 17 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 2150-7511 J9 MBIO JI mBio PD JAN-FEB PY 2013 VL 4 IS 1 AR e00516-12 DI 10.1128/mBio.00516-12 PG 1 WC Microbiology SC Microbiology GA 102AA UT WOS:000315814300021 ER PT J AU Chae, PS Wander, MJ Cho, KH Laible, PD Gellman, SH AF Chae, Pil Seok Wander, Marc J. Cho, Kyung Ho Laible, Philip D. Gellman, Samuel H. TI Carbohydrate-containing Triton X-100 analogues for membrane protein solubilization and stabilization SO MOLECULAR BIOSYSTEMS LA English DT Article ID MUSCARINIC ACETYLCHOLINE-RECEPTOR; FACIAL AMPHIPHILES; AQUEOUS-SOLUTIONS; CARBON NANOTUBES; DETERGENT; SURFACTANTS; CRYSTALLIZATION; ADRENOCEPTOR; ANTAGONIST; AMPHIPOLS AB Membrane protein manipulation is a challenging task owing to limited tertiary and quaternary structural stability once the protein has been removed from a lipid bilayer. Such instability can be overcome by embedding membrane proteins in detergent micelles formed from amphiphiles with carefully tuned properties. This study introduces a class of easy-to-synthesize amphiphiles, which are designated CGT (Chae's Glyco-Triton) detergents. Some of the agents are well suited for membrane protein solubilization and stabilization. C1 [Chae, Pil Seok; Cho, Kyung Ho] Hanyang Univ, Dept Bionano Engn, Ansan 426791, South Korea. [Wander, Marc J.; Laible, Philip D.] Argonne Natl Lab, Biosci Div, Argonne, IL 60439 USA. [Gellman, Samuel H.] Univ Wisconsin, Dept Chem, Madison, WI 53706 USA. RP Chae, PS (reprint author), Hanyang Univ, Dept Bionano Engn, Ansan 426791, South Korea. EM pchae@hanyang.ac.kr; laible@anl.gov; gellman@chem.wisc.edu FU National Research Foundation of Korea (NRF); Ministry of Education, Science and Technology [2008-0061856, 2012R1A1A1040964]; NIH grant [P01 GM75913] FX This research was supported by the National Research Foundation of Korea (NRF) funded by the Ministry of Education, Science and Technology (grant number 2008-0061856 and 2012R1A1A1040964 to P.S.C., K.H.C.), and NIH grant P01 GM75913 (S.H.G., P.D.L., M.J.W). NR 56 TC 11 Z9 11 U1 1 U2 21 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1742-206X EI 1742-2051 J9 MOL BIOSYST JI Mol. Biosyst. PY 2013 VL 9 IS 4 BP 626 EP 629 DI 10.1039/c3mb25584k PG 4 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA 103IG UT WOS:000315908800012 PM 23377371 ER PT J AU Bhattacharya, P Geitner, NK Sarupria, S Ke, PC AF Bhattacharya, Priyanka Geitner, Nicholas K. Sarupria, Sapna Ke, Pu Chun TI Exploiting the physicochemical properties of dendritic polymers for environmental and biological applications SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Editorial Material ID SUPPORTED LIPID-BILAYERS; POLYCYCLIC AROMATIC-HYDROCARBONS; MOLECULAR-DYNAMICS SIMULATIONS; POLY(AMIDOAMINE) DENDRIMERS; STARBURST DENDRIMERS; PAMAM DENDRIMERS; DRUG-DELIVERY; MACROMOLECULAR ARCHITECTURE; POLYAMIDOAMINE DENDRIMERS; HYPERBRANCHED POLYMERS AB In this perspective we first examine the rich physicochemical properties of dendritic polymers for hosting cations, anions, and polyaromatic hydrocarbons. We then extrapolate these conceptual discussions to the use of dendritic polymers in humic acid antifouling, oil dispersion, copper sensing, and fullerenol remediation. In addition, we review the state-of-the-art of dendrimer research and elaborate on its implications for water purification, environmental remediation, nanomedicine, and energy harvesting. C1 [Bhattacharya, Priyanka] Pacific NW Natl Lab, Richland, WA 99352 USA. [Geitner, Nicholas K.; Ke, Pu Chun] Clemson Univ, COMSET, Nanobiophys & Soft Matter Lab, Clemson, SC 29634 USA. [Sarupria, Sapna] Clemson Univ, Dept Chem & Biomol Engn, Clemson, SC 29634 USA. RP Bhattacharya, P (reprint author), Pacific NW Natl Lab, 902 Battelle Blvd,POB 999,MSIN K2-44, Richland, WA 99352 USA. EM priyanka.bhattacharya@pnnl.gov; pcke11@clemson.edu RI Ke, Pu Chun/A-9378-2008; Ke, Pu Chun /K-2805-2013; Bhattacharya, Priyanka/E-1652-2011; OI Ke, Pu Chun /0000-0001-9825-3302; Bhattacharya, Priyanka/0000-0003-0368-8480; Geitner, Nicholas/0000-0003-4313-372X NR 122 TC 13 Z9 14 U1 7 U2 69 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PY 2013 VL 15 IS 13 BP 4477 EP 4490 DI 10.1039/c3cp44591g PG 14 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 099VA UT WOS:000315649500002 PM 23400225 ER PT J AU Kumar, R Goswami, M Sumpter, BG Novikov, VN Sokolov, AP AF Kumar, Rajeev Goswami, Monojoy Sumpter, Bobby G. Novikov, Vladimir N. Sokolov, Alexei P. TI Effects of backbone rigidity on the local structure and dynamics in polymer melts and glasses SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID FREE-VOLUME DISTRIBUTION; MOLECULAR-DYNAMICS; TRANSITION TEMPERATURE; COMPUTER-SIMULATION; CHEMICAL-STRUCTURE; LIQUID; ELECTROLYTES; RELAXATION; CELLS; DISTRIBUTIONS AB Frustration in chain packing has been proposed to play an important role in thermodynamic and dynamic properties of polymeric melts and glasses. Based on a quantitative analysis using Voronoi tessellations and large scale molecular dynamics simulations of flexible and semi-flexible polymers, we demonstrate that the rigid polymer chains have higher averaged Voronoi polyhedral volumes and significantly wider distribution of the volume due to frustration in the chain packing. Using these results, we discuss the advantage of the rigid polymers for possible enhancement of transport properties, e.g. for enhancing ionic conductivity in solid polymer electrolytes. C1 [Kumar, Rajeev] Oak Ridge Natl Lab, Natl Ctr Computat Sci, Oak Ridge, TN 37831 USA. [Goswami, Monojoy] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. [Sumpter, Bobby G.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Novikov, Vladimir N.; Sokolov, Alexei P.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Novikov, Vladimir N.; Sokolov, Alexei P.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. RP Kumar, R (reprint author), Oak Ridge Natl Lab, Natl Ctr Computat Sci, Oak Ridge, TN 37831 USA. EM kumarr@ornl.gov RI Sumpter, Bobby/C-9459-2013; KUMAR, RAJEEV/D-2562-2010; Kumar, Rajeev/Q-2255-2015; Goswami, Monojoy/G-7943-2012 OI Sumpter, Bobby/0000-0001-6341-0355; Kumar, Rajeev/0000-0001-9494-3488; Goswami, Monojoy/0000-0002-4473-4888 FU Division of Materials Science and Engineering, U.S. Department of Energy, Office of Basic Energy Sciences; Oak Ridge Leadership Computing Facility at the Oak Ridge National Laboratory; Office of Science of the U.S. Department of Energy [DE-AC05-00OR22725]; UT-Battelle through the LDRD program [05608] FX MG, BGS and APS acknowledge financial support from the Division of Materials Science and Engineering, U.S. Department of Energy, Office of Basic Energy Sciences. RK acknowledges support from the Oak Ridge Leadership Computing Facility at the Oak Ridge National Laboratory, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC05-00OR22725. Also, we acknowledge support from UT-Battelle through the LDRD program (project #05608) during initial stages of this work. NR 55 TC 22 Z9 22 U1 1 U2 74 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PY 2013 VL 15 IS 13 BP 4604 EP 4609 DI 10.1039/c3cp43737j PG 6 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 099VA UT WOS:000315649500018 PM 23423355 ER PT J AU Miller, JA Klippenstein, SJ AF Miller, James A. Klippenstein, Stephen J. TI Determining phenomenological rate coefficients from a time-dependent, multiple-well master equation: "species reduction" at high temperatures SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID THERMAL-ACTIVATION REACTIONS; REVERSIBLE ISOMERIZATION; UNIMOLECULAR REACTIONS; BIMOLECULAR REACTIONS; CHEMICAL-REACTIONS; ENERGY-TRANSFER; RADICALS; DECOMPOSITION; RECOMBINATION; THRESHOLDS AB In this article we discuss at length the determination of phenomenological rate coefficients from the solution to a time-dependent, multiple-well master equation. Both conservative and non-conservative formulations are considered. The emphasis is placed on how to handle the situation when a CSE (chemically significant eigenvalue of the transition matrix) merges with the quasi-continuum of IEREs (internal energy relaxation eigenvalues), indicating that one or more chemical reactions begin to take place on vibrational-rotational relaxation time scales. The methodology is illustrated with four examples. C1 [Miller, James A.; Klippenstein, Stephen J.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Miller, JA (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM jamiller@anl.gov OI Klippenstein, Stephen/0000-0001-6297-9187 FU Division of Chemical Sciences, Geosciences, and Biosciences, the Office of Basic Energy Sciences, the U.S. Department of Energy [DE-AC02-2006CH11357]; Division of Chemical Sciences, Geosciences, and Biosciences, the Office of Basic Energy Sciences, the U.S. Department of Energy as part of the ASC-HPCC (ANL FWP) [59044] FX This work was supported by the Division of Chemical Sciences, Geosciences, and Biosciences, the Office of Basic Energy Sciences, the U.S. Department of Energy, under contract number DE-AC02-2006CH11357 as part of the ASC-HPCC (ANL FWP # 59044). NR 33 TC 15 Z9 16 U1 0 U2 39 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PY 2013 VL 15 IS 13 BP 4744 EP 4753 DI 10.1039/c3cp44337j PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 099VA UT WOS:000315649500035 PM 23435763 ER PT J AU Jiao, Y Du, AJ Hankel, M Smith, SC AF Jiao, Yan Du, Aijun Hankel, Marlies Smith, Sean C. TI Modelling carbon membranes for gas and isotope separation SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID SINGLE-WALLED CARBON; TRANSITION-STATE THEORY; CENTROID MOLECULAR-DYNAMICS; MONTE-CARLO SIMULATIONS; LENNARD-JONES FLUIDS; POROUS GRAPHENE; HYDROGEN PURIFICATION; NANOTUBE MEMBRANES; SILICA MEMBRANES; NANOPOROUS GRAPHENE AB Molecular modelling has become a useful and widely applied tool to investigate separation and diffusion behavior of gas molecules through nano-porous low dimensional carbon materials, including quasi-1D carbon nanotubes and 2D graphene-like carbon allotropes. These simulations provide detailed, molecular level information about the carbon framework structure as well as dynamics and mechanistic insights, i.e. size sieving, quantum sieving, and chemical affinity sieving. In this perspective, we revisit recent advances in this field and summarize separation mechanisms for multicomponent systems from kinetic and equilibrium molecular simulations, elucidating also anomalous diffusion effects induced by the confining pore structure and outlining perspectives for future directions in this field. C1 [Jiao, Yan; Hankel, Marlies] Univ Queensland, Australian Inst Bioengn & Nanotechnol, Ctr Computat Mol Sci, Brisbane, Qld 4072, Australia. [Jiao, Yan] Univ Adelaide, Sch Chem Engn, Adelaide, SA 5005, Australia. [Du, Aijun] Queensland Univ Technol, Sch Chem Phys & Mech Engn, Brisbane, Qld 4001, Australia. [Smith, Sean C.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Smith, SC (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM smithsc@ornl.gov RI Jiao, Yan/J-5322-2012; Hankel, Marlies/C-6262-2009; Smith, Sean/H-5003-2015; Du, Aijun/C-5759-2009 OI Jiao, Yan/0000-0003-1329-4290; Hankel, Marlies/0000-0002-8297-7231; Smith, Sean/0000-0002-5679-8205; Du, Aijun/0000-0002-3369-3283 FU Center for Nanophase Materials Sciences; Scientific User Facilities Division, Basic Energy Sciences, US Department of Energy FX We acknowledge generous grants of high performance computer time from the CCMS/AIBN cluster computing facility and QCIF at The University of Queensland and the Australian NCI facility. S.C.S. acknowledges support from the Center for Nanophase Materials Sciences, which is sponsored at the Oak Ridge National Laboratory by the Scientific User Facilities Division, Basic Energy Sciences, US Department of Energy. NR 132 TC 35 Z9 35 U1 9 U2 166 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PY 2013 VL 15 IS 14 BP 4832 EP 4843 DI 10.1039/c3cp44414g PG 12 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 104PX UT WOS:000316007900001 PM 23348369 ER PT J AU Chang, Y Brunello, GF Fuller, J Disabb-Miller, ML Hawley, ME Kim, YS Hickner, MA Jang, SS Bae, C AF Chang, Ying Brunello, Giuseppe F. Fuller, Jeffrey Disabb-Miller, Melanie L. Hawley, Marilyn E. Kim, Yu Seung Hickner, Michael A. Jang, Seung Soon Bae, Chulsung TI Polymer electrolyte membranes based on poly(arylene ether sulfone) with pendant perfluorosulfonic acid SO POLYMER CHEMISTRY LA English DT Article ID PROTON-EXCHANGE MEMBRANES; MONTE-CARLO-SIMULATION; FUEL-CELL APPLICATIONS; C-H BONDS; NANOPHASE-SEGREGATION; AROMATIC IONOMERS; PERFORMANCE; ACTIVATION; COPOLYMERS; TRANSPORT AB Poly(arylene ether sulfone)-based ionomers with sulfonate groups of varying acidity (perfluoroalkyl sulfonate, aryl sulfonate and alkyl sulfonate) were synthesized via borylation of aromatic C-H bonds and Suzuki coupling with sulfonated phenyl bromides. Properties of the ionomers, such as thermal stability, water uptake, ion exchange capacity, morphology and proton conductivity, were analyzed with respect to the effect of the sulfonate group. Superacidic fluoroalkyl sulfonated ionomers displayed much higher conductivity at low relative humidity than less acidic aryl and alkyl sulfonated ionomers in spite of their lower ion exchange capacities. The water uptake of the membranes correlated with their IEC, regardless of the acid group identity. The membranes with fluoroalkyl and alkyl sulfonate groups had similar hydration numbers as a function of RH, but the hydration number of the aromatic sulfonate sample was greater than the other polymers. Ionic domain structure analysis by atomic force microscopy, transmission electron microscopy and small-angle X-ray scattering revealed that all of the aromatic ionomers in this study had a small, disorganized phase structure. These results demonstrate that the primary influence on the proton conductivity of these randomly sulfonated copolymers is the acid strength while the nanoscale domain structure plays a secondary role in the low RH proton transport. C1 [Disabb-Miller, Melanie L.; Hickner, Michael A.] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. [Chang, Ying; Bae, Chulsung] Rensselaer Polytech Inst, New York State Ctr Polymer Synth, Dept Chem & Chem Biol, Troy, NY 12180 USA. [Chang, Ying; Bae, Chulsung] Univ Nevada Las Vegas, Dept Chem, Las Vegas, NV 89154 USA. [Brunello, Giuseppe F.; Fuller, Jeffrey; Jang, Seung Soon] Georgia Inst Technol, Sch Mat Sci & Engn, Atlanta, GA 30332 USA. [Hawley, Marilyn E.] Los Alamos Natl Lab, Polymers & Coating Grp, MST 7, Los Alamos, NM 87544 USA. [Kim, Yu Seung] Los Alamos Natl Lab, Sensors & Elect Devices Grp, MPA 11, Los Alamos, NM 87544 USA. RP Hickner, MA (reprint author), Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. EM Hickner@matse.psu.edu; seungsoon.jang@mse.gatech.edu; baec@rpi.edu RI Jang, Seung Soon/C-6847-2008 FU NSF; Nevada Renewable Energy Consortium; Rensselaer Polytechnic Institute; National Science Foundation [CBET-0803137]; Penn State Materials Research Institute; Penn State Institutes of Energy; Environment for infrastructure support; US DOE Fuel Cell Technologies Program; Technology Development Manager Dr Nancy Garland FX CB thanks the NSF (CAREER), Nevada Renewable Energy Consortium, and Rensselaer Polytechnic Institute for their generous support, Sinocompound for a donation of iridium and palladium catalyst, Frontier Scientific Co. for a gift of B2pin2, Dr Longzhou Ma of UNLV HRC for his help in running TEM. M. A. H. acknowledges the support of the National Science Foundation, Grant CBET-0803137, and the Penn State Materials Research Institute and Penn State Institutes of Energy and the Environment for infrastructure support. The authors at Los Alamos National Laboratory thank the US DOE Fuel Cell Technologies Program and Technology Development Manager Dr Nancy Garland for financial support. NR 38 TC 31 Z9 31 U1 5 U2 78 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1759-9954 J9 POLYM CHEM-UK JI Polym. Chem. PY 2013 VL 4 IS 2 BP 272 EP 281 DI 10.1039/c2py20666h PG 10 WC Polymer Science SC Polymer Science GA 052TO UT WOS:000312221600013 ER PT J AU Kale, S Peres, Y Seshadhri, C AF Kale, Satyen Peres, Yuval Seshadhri, C. TI NOISE TOLERANCE OF EXPANDERS AND SUBLINEAR EXPANSION RECONSTRUCTION SO SIAM JOURNAL ON COMPUTING LA English DT Article DE graph expansion; random walks; sublinear algorithms; sublinear reconstruction ID BOUNDED-DEGREE GRAPHS; APPROXIMATION; TESTER AB We consider the problem of online sublinear expander reconstruction and its relation to random walks in "noisy" expanders. Given access to an adjacency list representation of a bounded-degree graph G, we want to convert this graph into a bounded-degree expander G' changing G as little as possible. The graph G' will be output by a distributed filter: this is a sublinear time procedure that, given a query vertex, outputs all its neighbors in G' and can do so even in a distributed manner, ensuring consistency in all the answers. One of the main tools in our analysis is a result on the behavior of random walks in graph that are almost expanders: graphs that are formed by arbitrarily connecting a small unknown graph (the noise) to a large expander. We show that a random walk from almost any vertex in the expander part will have fast mixing properties, in the general setting of irreducible finite Markov chains. We also design sublinear time procedures to distinguish vertices of the expander part from those in the noise part and use this procedure in the reconstruction algorithm. C1 [Kale, Satyen] IBM TJ Watson Res Ctr, Yorktown Hts, NY 10598 USA. [Kale, Satyen; Peres, Yuval] Microsoft Res, Redmond, WA 98052 USA. [Seshadhri, C.] Sandia Natl Labs, Livermore, CA 94550 USA. [Seshadhri, C.] Princeton Univ, Princeton, NJ 08544 USA. RP Kale, S (reprint author), IBM TJ Watson Res Ctr, POB 218, Yorktown Hts, NY 10598 USA. EM sckale@us.ibm.com; peres@microsoft.com; scomand@sandia.gov FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was done when the author was at Princeton University and IBM Almaden Research Center. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 29 TC 0 Z9 0 U1 0 U2 1 PU SIAM PUBLICATIONS PI PHILADELPHIA PA 3600 UNIV CITY SCIENCE CENTER, PHILADELPHIA, PA 19104-2688 USA SN 0097-5397 J9 SIAM J COMPUT JI SIAM J. Comput. PY 2013 VL 42 IS 1 BP 305 EP 323 DI 10.1137/110837863 PG 19 WC Computer Science, Theory & Methods; Mathematics, Applied SC Computer Science; Mathematics GA 098WF UT WOS:000315579100012 ER PT J AU Pencheva, GV Vohralik, M Wheeler, MF Wildey, T AF Pencheva, Gergina V. Vohralik, Martin Wheeler, Mary F. Wildey, Tim TI ROBUST A POSTERIORI ERROR CONTROL AND ADAPTIVITY FOR MULTISCALE, MULTINUMERICS, AND MORTAR COUPLING SO SIAM JOURNAL ON NUMERICAL ANALYSIS LA English DT Article DE multiscale; multinumerics; mortar coupling; nonmatching grids; a posteriori error estimate; guaranteed upper bound; robustness; balancing error components ID FINITE-ELEMENT METHODS; LOCALLY CONSERVATIVE METHODS; 2ND-ORDER ELLIPTIC PROBLEMS; DISCONTINUOUS GALERKIN; FLUX RECONSTRUCTION; POROUS-MEDIA; VOLUME; DISCRETIZATIONS; APPROXIMATIONS; EQUATIONS AB We consider discretizations of a model elliptic problem by means of different numerical methods applied separately in different subdomains, termed multinumerics, coupled using the mortar technique. The grids need not match along the interfaces. We are also interested in the multiscale setting, where the subdomains are partitioned by a mesh of size h, whereas the interfaces are partitioned by a mesh of much coarser size H, and where lower-order polynomials are used in the subdomains and higher-order polynomials are used on the mortar interface mesh. We derive several fully computable a posteriori error estimates which deliver a guaranteed upper bound on the error measured in the energy norm. Our estimates are also locally efficient and one of them is robust with respect to the ratio H/h under an assumption of sufficient regularity of the weak solution. The present approach allows bounding separately and comparing mutually the subdomain and interface errors. A subdomain/interface adaptive refinement strategy is proposed and numerically tested. C1 [Pencheva, Gergina V.; Wheeler, Mary F.] Univ Texas Austin, Inst Computat Engn & Sci, Austin, TX 78712 USA. [Vohralik, Martin] Univ Paris 06, UMR 7598, Lab Jacques Louis Lions, F-75005 Paris, France. [Vohralik, Martin] CNRS, UMR 7598, Lab Jacques Louis Lions, F-75005 Paris, France. [Wildey, Tim] Sandia Natl Labs, Optimizat & Uncertainty Quantificat Dept, Albuquerque, NM 87185 USA. RP Pencheva, GV (reprint author), Univ Texas Austin, Inst Computat Engn & Sci, Austin, TX 78712 USA. EM gergina@ices.utexas.edu; martin.vohralik@inria.fr; mfw@ices.utexas.edu; tmwilde@sandia.gov FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences; Center for Frontiers of Subsurface Energy Security (CFSES) is a DOE Energy Frontier Research Center [DE-SC0001114]; NSF-CDI [DMS 0835745]; King Abdullah University of Science and Technology [(KAUST)-AEA-UTA08-687]; DOE [DE-FGO2-04ER25617]; GNR MoMaS project "Numerical Simulations and Mathematical Modeling of Underground Nuclear Waste Disposal"; PACEN/CNRS; ANDRA; BRGM; CEA; EdF; IRSN, France; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX A portion of this research was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. The Center for Frontiers of Subsurface Energy Security (CFSES) is a DOE Energy Frontier Research Center, under Award Number DE-SC0001114. The authors gratefully acknowledge the financial support provided by the NSF-CDI under contract DMS 0835745 and King Abdullah University of Science and Technology (KAUST)-AEA-UTA08-687 and DOE grant DE-FGO2-04ER25617.; This author was supported by the GNR MoMaS project "Numerical Simulations and Mathematical Modeling of Underground Nuclear Waste Disposal," PACEN/CNRS, ANDRA, BRGM, CEA, EdF, IRSN, France.; Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 39 TC 6 Z9 6 U1 0 U2 4 PU SIAM PUBLICATIONS PI PHILADELPHIA PA 3600 UNIV CITY SCIENCE CENTER, PHILADELPHIA, PA 19104-2688 USA SN 0036-1429 J9 SIAM J NUMER ANAL JI SIAM J. Numer. Anal. PY 2013 VL 51 IS 1 BP 526 EP 554 DI 10.1137/110839047 PG 29 WC Mathematics, Applied SC Mathematics GA 098UD UT WOS:000315573700025 ER PT J AU Dobnikar, J Snezhko, A Yethiraj, A AF Dobnikar, Jure Snezhko, Alexey Yethiraj, Anand TI Emergent colloidal dynamics in electromagnetic fields SO SOFT MATTER LA English DT Review ID ELECTRORHEOLOGICAL FLUIDS; ELECTRIC-FIELD; STRUCTURED COMPOSITES; BIAXIAL FIELD; ROD-LIKE; MODEL; ELECTROHYDRODYNAMICS; PARTICLES; DIPOLAR; TRANSITIONS AB We present a current review of the collective dynamics that can arise in colloidal systems subjected to electromagnetic fields. The focus is on phenomena that are not simply understandable purely from a dipolar model, but instead emerge from the collective behavior of many discrete interacting components driven out of equilibrium by external forces. We examine in particular the fascinating diversity of large-scale dynamical structures that arise due to the interplay between the induced interactions, time-dependent energy injection, and coupling with the fluid flow. C1 [Dobnikar, Jure] Univ Cambridge, Dept Chem, Cambridge CB2 1EW, England. [Dobnikar, Jure] Jozef Stefan Inst, Dept Theoret Phys, Ljubljana 1000, Slovenia. [Snezhko, Alexey] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Yethiraj, Anand] Mem Univ Newfoundland, Dept Phys & Phys Oceanog, St John, NF A1B 3X7, Canada. RP Dobnikar, J (reprint author), Univ Cambridge, Dept Chem, Lensfield Rd, Cambridge CB2 1EW, England. EM jd489@cam.ac.uk; snezhko@anl.gov; ayethiraj@mun.ca RI Dobnikar, Jure/C-8765-2011; Yethiraj, Anand/L-4325-2014 OI Dobnikar, Jure/0000-0002-1169-6619; Yethiraj, Anand/0000-0003-1293-2801 FU CECAM; European Union [ITN-COMPLOIDS 234810, ARG-ERC-COLSTRUCTION 227758]; U.S. DOE, Office of Basic Energy Sciences, Division of Materials Science and Engineering [DE AC02-06CH11357]; Slovenian research agency [P1-0055]; National Science and Engineering Research Council of Canada (NSERC) FX We acknowledge the support of CECAM and of 7th Framework Program of European Union (ITN-COMPLOIDS 234810), who co-sponsored the workshop on Emergent Dynamics in Driven Colloids held in Lausanne, 26-28.4.2012 (http://www.cecam.org/workshop-690.html). A.S. acknowledges the support of the U.S. DOE, Office of Basic Energy Sciences, Division of Materials Science and Engineering, under the Contract no. DE AC02-06CH11357. J.D. acknowledges the support of the 7th Framework Program of European Union through grants ARG-ERC-COLSTRUCTION 227758 and ITN-COMPLOIDS 234810, and by the Slovenian research agency through Grant P1-0055. A.Y. acknowledges financial support from the National Science and Engineering Research Council of Canada (NSERC) as well as the hospitality of the groups of Profs. Stefan Egelhaaf and Juergen Horbach at Heinrich Heine University, Duesseldorf. NR 90 TC 39 Z9 39 U1 1 U2 65 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1744-683X EI 1744-6848 J9 SOFT MATTER JI Soft Matter PY 2013 VL 9 IS 14 BP 3693 EP 3704 DI 10.1039/c3sm27363f PG 12 WC Chemistry, Physical; Materials Science, Multidisciplinary; Physics, Multidisciplinary; Polymer Science SC Chemistry; Materials Science; Physics; Polymer Science GA 106CF UT WOS:000316118300001 ER PT J AU Ewing, RG Waltman, MJ Atkinson, DA Grate, JW Hotchkiss, PJ AF Ewing, Robert G. Waltman, Melanie J. Atkinson, David A. Grate, Jay W. Hotchkiss, Peter J. TI The vapor pressures of explosives SO TRAC-TRENDS IN ANALYTICAL CHEMISTRY LA English DT Article DE Direct vapor detection; Explosive; NG; Particle-based detection; PETN; RDX; Security; TNT; Vapor pressure; Vapor-pressure equation ID ETHYLENE-GLYCOL DINITRATE; HEADSPACE TECHNIQUE; CANINE DETECTION; SUBLIMATION; 2,4,6-TRINITROTOLUENE; NITROGLYCERIN; SPECTROMETRY; TETRANITRATE; TRINITRATE; PEROXIDE AB The vapor pressures (VPs) of many explosive compounds are extremely low, so determining accurate values proves difficult. Many researchers, using a variety of methods, have measured and reported the VPs of explosive compounds at single temperatures, or as a function of temperature using VP equations. There are large variations in reported VPs for many of these compounds, and some errors exist within individual papers. This article provides a review of explosive VPs and describes the methods used to determine them. We have compiled primary VP relationships traceable to the original citations and include the temperature ranges for which they have been determined. Corrected values are reported as needed and described in the text. In addition, after critically examining the available data, we calculate and tabulate VPs at 25 degrees C. (c) 2012 Elsevier Ltd. All rights reserved. C1 [Ewing, Robert G.; Waltman, Melanie J.; Atkinson, David A.; Grate, Jay W.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Hotchkiss, Peter J.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Ewing, RG (reprint author), Pacific NW Natl Lab, POB 999, Richland, WA 99352 USA. EM robert.ewing@pnnl.gov FU David Jones; Laboratory Directed Research and Development funding at Pacific Northwest National Laboratory FX We acknowledge Joda Wormhoudt for providing information of Colin Wood's Thesis and Colin Wood for supplying raw data from his Thesis/Dissertation. PJH acknowledges David Jones for partial funding. This work was funded in part by Laboratory Directed Research and Development funding at Pacific Northwest National Laboratory, which is a multiprogram national laboratory operated for the US Department of Energy by Battelle Memorial Institute. NR 71 TC 48 Z9 48 U1 8 U2 89 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0165-9936 J9 TRAC-TREND ANAL CHEM JI Trac-Trends Anal. Chem. PD JAN PY 2013 VL 42 BP 35 EP 48 DI 10.1016/j.trac.2012.09.010 PG 14 WC Chemistry, Analytical SC Chemistry GA 099FR UT WOS:000315607400013 ER PT S AU Bayes, R Bross, A Cervera-Villanueva, A Ellis, M Laing, A Soler, FJP Wands, R AF Bayes, R. Bross, A. Cervera-Villanueva, A. Ellis, M. Laing, A. Soler, F. J. P. Wands, R. BE Blondel, A Efthymiopoulos, I Prior, G TI Status of a MIND type Neutrino Factory Far Detector SO XIII INTERNATIONAL WORKSHOP ON NEUTRINO FACTORIES, SUPER BEAMS AND BETA BEAMS (NUFACT11) SE Journal of Physics Conference Series LA English DT Proceedings Paper CT 13th International Workshop on Neutrino Factories, Super beams and Beta beams (NUFACT) CY AUG 01-06, 2011 CL Geneva, SWITZERLAND SP European Org Nucl Res (CERN), Univ Geneva, Swiss Inst Particle Phys (CHIPP), European FP7 mandate EuCARD ID MONTE-CARLO GENERATOR; RECONSTRUCTION; SIMULATION AB A realistic simulation and analysis of a Magnetized Iron Neutrino Detector (MIND) has been developed for the purpose of understanding the potential sensitivity of such a facility. The status of the MIND simulation and reconstruction as discussed in the interim design report is reviewed here. Priorities for producing a more realistic simulation for a reference design report will be discussed, as will be the steps that have already been taken towards an improved simulation. C1 [Bayes, R.; Laing, A.; Soler, F. J. P.] Univ Glasgow, Sch Phys & Astron, Glasgow G12 8QQ, Lanark, Scotland. [Cervera-Villanueva, A.] Univ Valencia, Valencia, Spain. [Cervera-Villanueva, A.] IFIC, Valencia, Spain. [Bross, A.; Wands, R.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Ellis, M.] Brunell Univ West London, Uxbridge UB8 3PH, Middx, England. [Ellis, M.] Westpac Inst Bank, Sydney, NSW, Australia. RP Bayes, R (reprint author), Univ Glasgow, Sch Phys & Astron, Glasgow G12 8QQ, Lanark, Scotland. EM Ryan.Bayes@glasgow.ac.uk RI Soler, Paul/E-8464-2011 OI Soler, Paul/0000-0002-4893-3729 NR 9 TC 1 Z9 1 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA DIRAC HOUSE, TEMPLE BACK, BRISTOL BS1 6BE, ENGLAND SN 1742-6588 J9 J PHYS CONF SER PY 2013 VL 408 AR 012075 DI 10.1088/1742-6596/408/1/012075 PG 4 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA BDW66 UT WOS:000315385900075 ER PT S AU Beard, KB Bogacz, SA Morozov, VS Roblin, YR AF Beard, K. B. Bogacz, S. A. Morozov, V. S. Roblin, Y. R. BE Blondel, A Efthymiopoulos, I Prior, G TI Muon RLA - design status and simulations SO XIII INTERNATIONAL WORKSHOP ON NEUTRINO FACTORIES, SUPER BEAMS AND BETA BEAMS (NUFACT11) SE Journal of Physics Conference Series LA English DT Proceedings Paper CT 13th International Workshop on Neutrino Factories, Super beams and Beta beams (NUFACT) CY AUG 01-06, 2011 CL Geneva, SWITZERLAND SP European Org Nucl Res (CERN), Univ Geneva, Swiss Inst Particle Phys (CHIPP), European FP7 mandate EuCARD AB The Neutrino Factory baseline design involves a complex chain of accelerators beginning with a linac. This first pre-linac follows the capture and bunching section and accelerates the muons from about 244 to 900 MeV and must accept a high emittance beam about 30 cm wide with a 10% energy spread. It uses counterwound, shielded superconducting solenoids and 201 MHz superconducting cavities, and currently consists of 24 3 m and 24 5 m long cryomodules. The next stage is a 1st dogbone-shaped RLA that takes the total energy from 900 MeV to 3.6 GeV in 4.5 passes, followed by a 2nd RLA that takes the energy from 3.6 to 12.6 GeV in 4.5 passes. Simulations are in progress to optimize the optics and determine the radiation loads from beam loss and muon decay. C1 [Beard, K. B.] Muons Inc, Batavia, IL USA. [Bogacz, S. A.; Morozov, V. S.; Roblin, Y. R.] Jefferson Lab, Newport News, VA USA. RP Beard, KB (reprint author), Muons Inc, Batavia, IL USA. EM beard@muonsinc.com NR 5 TC 0 Z9 0 U1 0 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA DIRAC HOUSE, TEMPLE BACK, BRISTOL BS1 6BE, ENGLAND SN 1742-6588 J9 J PHYS CONF SER PY 2013 VL 408 AR 012066 DI 10.1088/1742-6596/408/1/012066 PG 4 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA BDW66 UT WOS:000315385900066 ER PT S AU Childress, S Strait, J AF Childress, S. Strait, J. BE Blondel, A Efthymiopoulos, I Prior, G TI Long baseline neutrino beams at Fermilab SO XIII INTERNATIONAL WORKSHOP ON NEUTRINO FACTORIES, SUPER BEAMS AND BETA BEAMS (NUFACT11) SE Journal of Physics Conference Series LA English DT Proceedings Paper CT 13th International Workshop on Neutrino Factories, Super beams and Beta beams (NUFACT) CY AUG 01-06, 2011 CL Geneva, SWITZERLAND SP European Org Nucl Res (CERN), Univ Geneva, Swiss Inst Particle Phys (CHIPP), European FP7 mandate EuCARD AB Fermilab has had a very active long baseline neutrino program since initiation of the NuMI project in 1998. Commissioned in 2005, the NuMI beam with 400 kW design power has been in operation for the MINOS neutrino oscillation program since that time. Upgrade of NuMI to 700 kW for NOvA is now well advanced, with implementation of the beam upgrades to be accomplished in 2012-2013. Design development for the next generation LBNE neutrino beam is now a major ongoing effort. We report here salient features and constraints for each of these beams, as well as significant challenges both experienced and expected. C1 [Childress, S.; Strait, J.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. RP Childress, S (reprint author), Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. EM childress@fnal.gov; strait@fnal.gov NR 5 TC 3 Z9 3 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA DIRAC HOUSE, TEMPLE BACK, BRISTOL BS1 6BE, ENGLAND SN 1742-6588 J9 J PHYS CONF SER PY 2013 VL 408 AR 012007 DI 10.1088/1742-6596/408/1/012007 PG 8 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA BDW66 UT WOS:000315385900007 ER PT S AU Djurcic, Z AF Djurcic, Zelimir BE Blondel, A Efthymiopoulos, I Prior, G TI Review of reactor antineutrino experiments SO XIII INTERNATIONAL WORKSHOP ON NEUTRINO FACTORIES, SUPER BEAMS AND BETA BEAMS (NUFACT11) SE Journal of Physics Conference Series LA English DT Proceedings Paper CT 13th International Workshop on Neutrino Factories, Super beams and Beta beams (NUFACT) CY AUG 01-06, 2011 CL Geneva, SWITZERLAND SP European Org Nucl Res (CERN), Univ Geneva, Swiss Inst Particle Phys (CHIPP), European FP7 mandate EuCARD ID NEUTRON FISSION-PRODUCTS; NUCLEAR-REACTOR; OSCILLATIONS; SPECTRA; MASSES AB As discussed elsewhere, the measurement of a non-zero value for theta(13) would open up a wide range of possibilities to explore CP-violation and the mass hierarchy. Experimental methods to measure currently the unknown mixing angle theta(13) include accelerator searches for the nu(e) appearance and precise measurements of reactor antineutrino disappearance. The reactor antineutrino experiments are designed to search for a non-vanishing mixing angle theta(13) with unprecedented sensitivity. This document describes current reactor antineutrino experiments and synergy between accelerator searches for the nu(e) appearance and precise measurements of reactor antineutrino disappearance. C1 Argonne Natl Lab, Argonne, IL 60439 USA. RP Djurcic, Z (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. EM zdjurcic@hep.anl.gov NR 65 TC 0 Z9 0 U1 0 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA DIRAC HOUSE, TEMPLE BACK, BRISTOL BS1 6BE, ENGLAND SN 1742-6588 J9 J PHYS CONF SER PY 2013 VL 408 AR 012008 DI 10.1088/1742-6596/408/1/012008 PG 8 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA BDW66 UT WOS:000315385900008 ER PT S AU Djurcic, Z AF Djurcic, Zelimir BE Blondel, A Efthymiopoulos, I Prior, G TI MiniBooNE oscillation results 2011 SO XIII INTERNATIONAL WORKSHOP ON NEUTRINO FACTORIES, SUPER BEAMS AND BETA BEAMS (NUFACT11) SE Journal of Physics Conference Series LA English DT Proceedings Paper CT 13th International Workshop on Neutrino Factories, Super beams and Beta beams (NUFACT) CY AUG 01-06, 2011 CL Geneva, SWITZERLAND SP European Org Nucl Res (CERN), Univ Geneva, Swiss Inst Particle Phys (CHIPP), European FP7 mandate EuCARD ID LSND EXPERIMENT AB The MiniBooNE neutrino oscillation search experiment at Fermilab has recently updated results from a search for (nu) over bar (mu) -> (nu) over bar (e) oscillations, using a data sample corresponding to 8:58 x 10(20) protons on target in anti-neutrino mode. These high statistics results represent an increase in statistics of 52% compared to the results published in 2010. An excess of 57.7 +/- 28.5 events is observed in the energy range 200 MeV < E-nu < 3000 MeV. The data favor LSND-like nu(mu) -> nu(e) oscillations over a background only hypothesis at 91.1% confidence level in the energy range 475 < E nu <3000 Me C1 Argonne Natl Lab, Argonne, IL 60439 USA. RP Djurcic, Z (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. EM zdjurcic@hep.anl.gov NR 29 TC 0 Z9 0 U1 0 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA DIRAC HOUSE, TEMPLE BACK, BRISTOL BS1 6BE, ENGLAND SN 1742-6588 J9 J PHYS CONF SER PY 2013 VL 408 AR 012027 DI 10.1088/1742-6596/408/1/012027 PG 4 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA BDW66 UT WOS:000315385900027 ER PT S AU Garoby, R Gollwitzer, K Koseki, T Thomason, J AF Garoby, R. Gollwitzer, K. Koseki, T. Thomason, J. BE Blondel, A Efthymiopoulos, I Prior, G TI Proton drivers for neutrino beams and other high intensity applications SO XIII INTERNATIONAL WORKSHOP ON NEUTRINO FACTORIES, SUPER BEAMS AND BETA BEAMS (NUFACT11) SE Journal of Physics Conference Series LA English DT Proceedings Paper CT 13th International Workshop on Neutrino Factories, Super beams and Beta beams (NUFACT) CY AUG 01-06, 2011 CL Geneva, SWITZERLAND SP European Org Nucl Res (CERN), Univ Geneva, Swiss Inst Particle Phys (CHIPP), European FP7 mandate EuCARD AB CERN, Fermilab, J-PARC and RAL tentatively plan to have proton accelerators delivering multi-MW of beam power in view of enhancing their physics reach especially in the domain of neutrinos. These plans are described, together with their benefits for other applications. C1 [Garoby, R.] CERN, BE HDO, CH-1211 Geneva 23, Switzerland. [Gollwitzer, K.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Koseki, T.] J PARC, KEK & JAEA, Tokai, Ibaraki 3191195, Japan. [Thomason, J.] ISIS, STFC, Rutherford Appleton Lab, Harwell OX11 0QX, England. RP Garoby, R (reprint author), CERN, BE HDO, CH-1211 Geneva 23, Switzerland. NR 18 TC 0 Z9 0 U1 0 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA DIRAC HOUSE, TEMPLE BACK, BRISTOL BS1 6BE, ENGLAND SN 1742-6588 J9 J PHYS CONF SER PY 2013 VL 408 AR 012016 DI 10.1088/1742-6596/408/1/012016 PG 8 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA BDW66 UT WOS:000315385900016 ER PT S AU Lee, HS AF Lee, Hye-Sung BE Blondel, A Efthymiopoulos, I Prior, G TI Long-range interaction effects on neutrino oscillation SO XIII INTERNATIONAL WORKSHOP ON NEUTRINO FACTORIES, SUPER BEAMS AND BETA BEAMS (NUFACT11) SE Journal of Physics Conference Series LA English DT Proceedings Paper CT 13th International Workshop on Neutrino Factories, Super beams and Beta beams (NUFACT) CY AUG 01-06, 2011 CL Geneva, SWITZERLAND SP European Org Nucl Res (CERN), Univ Geneva, Swiss Inst Particle Phys (CHIPP), European FP7 mandate EuCARD ID FORCES AB Motivated by the recent anomaly in the muon neutrino and anti-muon neutrino disappearance experiments, we consider a long-range interaction with an extremely light gauge boson and extraordinarily weak coupling. A long-range interaction, consistent with current bounds, could have very pronounced effects on atmospheric neutrino disappearance that will be studied with the IceCube DeepCore array, currently in operation, and can have a significant effect on future high-precision long-baseline oscillation experiments. This invited talk was based on the paper with Hooman Davoudiasl and William Marciano [1]. C1 Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. RP Lee, HS (reprint author), Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. EM hlee@bnl.gov NR 16 TC 0 Z9 0 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA DIRAC HOUSE, TEMPLE BACK, BRISTOL BS1 6BE, ENGLAND SN 1742-6588 J9 J PHYS CONF SER PY 2013 VL 408 AR 012032 DI 10.1088/1742-6596/408/1/012032 PG 4 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA BDW66 UT WOS:000315385900032 ER PT S AU Li, DR DeMello, A Virostek, SP Zisman, MS AF Li, Derun DeMello, Allan Virostek, S. P. Zisman, Michael S. BE Blondel, A Efthymiopoulos, I Prior, G TI RF Cavity Processing and Testing Plan for MICE SO XIII INTERNATIONAL WORKSHOP ON NEUTRINO FACTORIES, SUPER BEAMS AND BETA BEAMS (NUFACT11) SE Journal of Physics Conference Series LA English DT Proceedings Paper CT 13th International Workshop on Neutrino Factories, Super beams and Beta beams (NUFACT) CY AUG 01-06, 2011 CL Geneva, SWITZERLAND SP European Org Nucl Res (CERN), Univ Geneva, Swiss Inst Particle Phys (CHIPP), European FP7 mandate EuCARD AB Fabrication status of the MICE RF cavities will be described. Design of a single-cavity vessel to test the cavities will be discussed, along with the plans for processing and testing the cavities. C1 [Li, Derun; Zisman, Michael S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Accelerator & Fus Res Div, Berkeley, CA 94720 USA. [DeMello, Allan; Virostek, S. P.] Lawrence Berkeley Natl Lab, Div Engn, Berkeley, CA 94720 USA. RP Li, DR (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Accelerator & Fus Res Div, Berkeley, CA 94720 USA. EM dli@lbl.gov FU Office of Science; Office of High Energy Physics; U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Director, Office of Science, Office of High Energy Physics, of the U.S. Department of Energy, under Contract No. DE-AC02-05CH11231. NR 0 TC 0 Z9 0 U1 0 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA DIRAC HOUSE, TEMPLE BACK, BRISTOL BS1 6BE, ENGLAND SN 1742-6588 J9 J PHYS CONF SER PY 2013 VL 408 AR 012065 DI 10.1088/1742-6596/408/1/012065 PG 4 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA BDW66 UT WOS:000315385900065 ER PT S AU Morfin, JG AF Morfin, Jorge G. BE Blondel, A Efthymiopoulos, I Prior, G TI How can we use neutrino nucleus interactions as a probe of the strong interaction? SO XIII INTERNATIONAL WORKSHOP ON NEUTRINO FACTORIES, SUPER BEAMS AND BETA BEAMS (NUFACT11) SE Journal of Physics Conference Series LA English DT Proceedings Paper CT 13th International Workshop on Neutrino Factories, Super beams and Beta beams (NUFACT) CY AUG 01-06, 2011 CL Geneva, SWITZERLAND SP European Org Nucl Res (CERN), Univ Geneva, Swiss Inst Particle Phys (CHIPP), European FP7 mandate EuCARD AB Neutrino scattering experiments have been studying QCD for around 40 years. An example of the more recent studies of QCD with neutrinos is the NuTeV v-Fe experiment at Fermilab. The problem the community faces in trying to study QCD with neutrino data is that there is no experimentally verified way to convert neutrino-nucleus (for example, Fe) results to the equivalent neutrino-nucleon values making it difficult to combine neutrino nucleus scattering data in QCD global fits to extract parton distribution functions. This is particularly significant since there are now indications that nuclear effects in neutrino nucleus interactions might be different than those measured in charged-lepton nucleus scattering. To better understand this situation, the MINERvA neutrino-nucleus scattering experiment at Fermilab, a collaboration of elementary-particle and nuclear physicists, is systematically studying neutrino nuclear effects off of He, C, O, Fe and Pb for a more thorough A-dependent study of nuclear PDFs and these correction factors. C1 Fermilab Natl Accelerator Lab, Particle Phys Div, Neutrino Dept, Batavia, IL 60510 USA. RP Morfin, JG (reprint author), Fermilab Natl Accelerator Lab, Particle Phys Div, Neutrino Dept, POB 500, Batavia, IL 60510 USA. EM morfin@fnal.gov NR 5 TC 1 Z9 1 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA DIRAC HOUSE, TEMPLE BACK, BRISTOL BS1 6BE, ENGLAND SN 1742-6588 J9 J PHYS CONF SER PY 2013 VL 408 AR 012054 DI 10.1088/1742-6596/408/1/012054 PG 4 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA BDW66 UT WOS:000315385900054 ER PT S AU Muether, M AF Muether, Mathew BE Blondel, A Efthymiopoulos, I Prior, G TI NO nu A detector technology with initial performance from the surface prototype SO XIII INTERNATIONAL WORKSHOP ON NEUTRINO FACTORIES, SUPER BEAMS AND BETA BEAMS (NUFACT11) SE Journal of Physics Conference Series LA English DT Proceedings Paper CT 13th International Workshop on Neutrino Factories, Super beams and Beta beams (NUFACT) CY AUG 01-06, 2011 CL Geneva, SWITZERLAND SP European Org Nucl Res (CERN), Univ Geneva, Swiss Inst Particle Phys (CHIPP), European FP7 mandate EuCARD AB NO nu A, the NuMI Off-Axis nu(e) Appearance experiment, will study nu(mu) -> nu(e) oscillations characterized by the mixing angle theta(13). Provided theta(13) is large enough, NO nu A may ultimately determine the ordering of the neutrino masses and measure CP violation in neutrino oscillations. A complementary pair of detectors will be constructed similar to 14 mrad off beam axis to optimize the energy profile of the neutrinos. This system consists of a surface based 14 kTon liquid scintillatior tracking volume located 810 km from the main injector source (NuMI) in Ash River, Minnesota and a smaller underground 222 Ton near detector at the Fermilab. The first neutrino signals at the Ash River Site are expected prior to the 2012 accelerator shutdown. In the meantime, a near detector surface prototype has been completed and neutrinos from two Fermilab sources have been observed using the same highly segmented PVC and liquid scintillator detector system that will be deployed in the full scale experiment. Design and initial performance characteristics of this prototype system are being fed back into the design for the full NO nu A program. C1 Fermilab Natl Accelerator Lab, Neutrino Dept, Batavia, IL 60510 USA. RP Muether, M (reprint author), Fermilab Natl Accelerator Lab, Neutrino Dept, POB 500 MS 220, Batavia, IL 60510 USA. EM muether@fnal.gov NR 6 TC 0 Z9 0 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA DIRAC HOUSE, TEMPLE BACK, BRISTOL BS1 6BE, ENGLAND SN 1742-6588 J9 J PHYS CONF SER PY 2013 VL 408 AR 012076 DI 10.1088/1742-6596/408/1/012076 PG 4 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA BDW66 UT WOS:000315385900076 ER PT S AU Nakamura, SX AF Nakamura, Satoshi X. BE Blondel, A Efthymiopoulos, I Prior, G TI Charged-current and neutral-current coherent pion productions - Theoretical status SO XIII INTERNATIONAL WORKSHOP ON NEUTRINO FACTORIES, SUPER BEAMS AND BETA BEAMS (NUFACT11) SE Journal of Physics Conference Series LA English DT Proceedings Paper CT 13th International Workshop on Neutrino Factories, Super beams and Beta beams (NUFACT) CY AUG 01-06, 2011 CL Geneva, SWITZERLAND SP European Org Nucl Res (CERN), Univ Geneva, Swiss Inst Particle Phys (CHIPP), European FP7 mandate EuCARD ID NEUTRINOS; ENERGY AB The CC and NC coherent pion productions have been studied with PCAC-based models and microscopic models. Current status of the theoretical studies is reviewed. C1 Jefferson Lab, Excited Baryon Anal Ctr, Newport News, VA 23606 USA. RP Nakamura, SX (reprint author), Jefferson Lab, Excited Baryon Anal Ctr, Newport News, VA 23606 USA. EM satoshi@jlab.org NR 27 TC 1 Z9 1 U1 0 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA DIRAC HOUSE, TEMPLE BACK, BRISTOL BS1 6BE, ENGLAND SN 1742-6588 J9 J PHYS CONF SER PY 2013 VL 408 AR 012043 DI 10.1088/1742-6596/408/1/012043 PG 4 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA BDW66 UT WOS:000315385900043 ER PT S AU Pasternak, J Aslaninejad, M Berg, JS Bliss, N Bontoiu, C Cordwell, M Witte, H Kelliher, D Machida, S AF Pasternak, J. Aslaninejad, M. Berg, J. Scott Bliss, N. Bontoiu, C. Cordwell, M. Witte, H. Kelliher, D. Machida, S. BE Blondel, A Efthymiopoulos, I Prior, G TI Recent developments on the muon Non-Scaling FFAG for the Neutrino Factory and its subsystems SO XIII INTERNATIONAL WORKSHOP ON NEUTRINO FACTORIES, SUPER BEAMS AND BETA BEAMS (NUFACT11) SE Journal of Physics Conference Series LA English DT Proceedings Paper CT 13th International Workshop on Neutrino Factories, Super beams and Beta beams (NUFACT) CY AUG 01-06, 2011 CL Geneva, SWITZERLAND SP European Org Nucl Res (CERN), Univ Geneva, Swiss Inst Particle Phys (CHIPP), European FP7 mandate EuCARD AB The current status and recent developments on the muon non-scaling FFAG for the Neutrino Factory studied in the framework of the EUROnu/IDS-NF projects are presented. Beam dynamics studies, including the process of acceleration, are discussed. A first pass at engineering for the layout of the ring cell is described. Progress of studies on the main machine subsystems is discussed. The future plans for the study are described. C1 [Pasternak, J.; Aslaninejad, M.; Bontoiu, C.] Imperial Coll London, London, England. [Pasternak, J.] Rutherford Appleton Lab, ISIS, STFC, UK, Rutherford, NJ USA. [Berg, J. Scott] BNL, Upton, NY 11973 USA. [Bliss, N.; Cordwell, M.] STFC, Dept Technol, Daresbury Lab, Daresbury, England. [Witte, H.] Univ Oxford, JAI, Oxford, England. [Kelliher, D.; Machida, S.] Rutherford Appleton Lab, ASTeC, STFC, Harwell OX11 0QX, Berks, England. RP Pasternak, J (reprint author), Imperial Coll London, London, England. EM j.pasternak@imperial.ac.uk RI Berg, Joseph/E-8371-2014; OI Berg, Joseph/0000-0002-5955-6973; Kelliher, David/0000-0001-9583-7804 NR 4 TC 0 Z9 0 U1 0 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA DIRAC HOUSE, TEMPLE BACK, BRISTOL BS1 6BE, ENGLAND SN 1742-6588 J9 J PHYS CONF SER PY 2013 VL 408 AR 012057 DI 10.1088/1742-6596/408/1/012057 PG 4 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA BDW66 UT WOS:000315385900057 ER PT S AU Yonehara, K AF Yonehara, Katsuya CA MTA Working Grp BE Blondel, A Efthymiopoulos, I Prior, G TI Recent progress of RF cavity study at Mucool Test Area SO XIII INTERNATIONAL WORKSHOP ON NEUTRINO FACTORIES, SUPER BEAMS AND BETA BEAMS (NUFACT11) SE Journal of Physics Conference Series LA English DT Proceedings Paper CT 13th International Workshop on Neutrino Factories, Super beams and Beta beams (NUFACT) CY AUG 01-06, 2011 CL Geneva, SWITZERLAND SP European Org Nucl Res (CERN), Univ Geneva, Swiss Inst Particle Phys (CHIPP), European FP7 mandate EuCARD AB In order to develop an RF cavity that is applicable for a muon beam cooling channel, a new facility, called Mucool Test Area (MTA) has been built at Fermilab. MTA is a unique facility whose purpose is to test RF cavities in various conditions. There are 201 and 805 MHz high power sources, a 4-Tesla solenoid magnet, a cryogenic system including a Helium liquifier, an explosion proof apparatus to operate gaseous/liquid Hydrogen, and a beam transport line to send an intense H-beam from the Fermilab Linac accelerator to the MTA hall. Recent activities at MTA will be discussed in this document. C1 [Yonehara, Katsuya; MTA Working Grp] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. RP Yonehara, K (reprint author), Fermilab Natl Accelerator Lab, MS 221,POB 500, Batavia, IL 60510 USA. EM yonehara@fnal.gov NR 8 TC 1 Z9 1 U1 0 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA DIRAC HOUSE, TEMPLE BACK, BRISTOL BS1 6BE, ENGLAND SN 1742-6588 J9 J PHYS CONF SER PY 2013 VL 408 AR 012062 DI 10.1088/1742-6596/408/1/012062 PG 4 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA BDW66 UT WOS:000315385900062 ER PT S AU Zisman, MS AF Zisman, Michael S. BE Blondel, A Efthymiopoulos, I Prior, G TI Accelerators for future neutrino facilities: strengths and challenges SO XIII INTERNATIONAL WORKSHOP ON NEUTRINO FACTORIES, SUPER BEAMS AND BETA BEAMS (NUFACT11) SE Journal of Physics Conference Series LA English DT Proceedings Paper CT 13th International Workshop on Neutrino Factories, Super beams and Beta beams (NUFACT) CY AUG 01-06, 2011 CL Geneva, SWITZERLAND SP European Org Nucl Res (CERN), Univ Geneva, Swiss Inst Particle Phys (CHIPP), European FP7 mandate EuCARD AB Several different ideas have been put forward for future neutrino facilities, including a high-power conventional neutrino beam (a "Superbeam" facility), a Beta Beam facility based on stored beta-unstable ion beams, and a Neutrino Factory based on stored muon beams. Each of these has its advantages and disadvantages, and these are described here. After briefly describing the physics context, the various options will be described and their respective strengths and challenges indicated. The supporting R&D programs will be briefly discussed and a few specific technical questions for each facility will be outlined. C1 Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Accelerator & Fus Res Div, Berkeley, CA 94720 USA. RP Zisman, MS (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Accelerator & Fus Res Div, Berkeley, CA 94720 USA. EM mszisman@lbl.gov NR 7 TC 0 Z9 0 U1 0 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA DIRAC HOUSE, TEMPLE BACK, BRISTOL BS1 6BE, ENGLAND SN 1742-6588 J9 J PHYS CONF SER PY 2013 VL 408 AR 012002 DI 10.1088/1742-6596/408/1/012002 PG 8 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA BDW66 UT WOS:000315385900002 ER PT J AU Stockmann, U Adams, MA Crawford, JW Field, DJ Henakaarchchi, N Jenkins, M Minasny, B McBratney, AB de Courcelles, VD Singh, K Wheeler, I Abbott, L Angers, DA Baldock, J Bird, M Brookes, PC Chenu, C Jastrow, JD Lal, R Lehmann, J O'Donnell, AG Parton, WJ Whitehead, D Zimmermann, M AF Stockmann, Uta Adams, Mark A. Crawford, John W. Field, Damien J. Henakaarchchi, Nilusha Jenkins, Meaghan Minasny, Budiman McBratney, Alex B. de Courcelles, Vivien de Remy Singh, Kanika Wheeler, Ichsani Abbott, Lynette Angers, Denis A. Baldock, Jeffrey Bird, Michael Brookes, Philip C. Chenu, Claire Jastrow, Julie D. Lal, Rattan Lehmann, Johannes O'Donnell, Anthony G. Parton, William J. Whitehead, David Zimmermann, Michael TI The knowns, known unknowns and unknowns of sequestration of soil organic carbon SO AGRICULTURE ECOSYSTEMS & ENVIRONMENT LA English DT Review DE Soil carbon sequestration; Soil carbon pools; Soil carbon modelling ID LAND-USE CHANGE; MICROBIAL COMMUNITY STRUCTURE; NATURAL C-13 ABUNDANCE; MATTER DYNAMICS; LITTER DECOMPOSITION; CLIMATE-CHANGE; NITROGEN MINERALIZATION; TEMPERATURE SENSITIVITY; ENVIRONMENTAL-CHANGE; AGRICULTURAL SOILS AB Soil contains approximately 2344 Gt (1 gigaton = 1 billion tonnes) of organic carbon globally and is the largest terrestrial pool of organic carbon. Small changes in the soil organic carbon stock could result in significant impacts on the atmospheric carbon concentration. The fluxes of soil organic carbon vary in response to a host of potential environmental and anthropogenic driving factors. Scientists worldwide are contemplating questions such as: 'What is the average net change in soil organic carbon due to environmental conditions or management practices?', 'How can soil organic carbon sequestration be enhanced to achieve some mitigation of atmospheric carbon dioxide?' and 'Will this secure soil quality?'. These questions are far reaching, because maintaining and improving the world's soil resource is imperative to providing sufficient food and fibre to a growing population. Additional challenges are expected through climate change and its potential to increase food shortages. This review highlights knowledge of the amount of carbon stored in soils globally, and the potential for carbon sequestration in soil. It also discusses successful methods and models used to determine and estimate carbon pools and fluxes. This knowledge and technology underpins decisions to protect the soil resource. (C) 2012 Elsevier B.V. All rights reserved. C1 [Stockmann, Uta; Adams, Mark A.; Crawford, John W.; Field, Damien J.; Henakaarchchi, Nilusha; Jenkins, Meaghan; Minasny, Budiman; McBratney, Alex B.; de Courcelles, Vivien de Remy; Singh, Kanika; Wheeler, Ichsani] Univ Sydney, Fac Agr & Environm, Eveleigh, NSW 2015, Australia. [Abbott, Lynette] Univ Western Australia, Sch Earth & Environm, Crawley, WA 6009, Australia. [Abbott, Lynette] Univ Western Australia, UWA Inst Agr M082, Crawley, WA 6009, Australia. [Angers, Denis A.] Agr & Agri Food Canada, Quebec City, PQ G1V 2J3, Canada. [Baldock, Jeffrey] CSIRO Land & Water & Sustainable Agr Flagship, Glen Osmond, SA 5064, Australia. [Bird, Michael] James Cook Univ, Sch Earth & Environm Sci, Cairns 4870, Australia. [Bird, Michael] James Cook Univ, Ctr Trop Environm & Sustainabil Sci, Cairns 4870, Australia. [Brookes, Philip C.] Rothamsted Res, Harpenden AL5 2JQ, Herts, England. [Chenu, Claire] AgroTechParis, Paris, France. [Jastrow, Julie D.] Argonne Natl Lab, Biosci Div, Argonne, IL 60439 USA. [Lal, Rattan] Ohio State Univ, Sch Environm & Nat Resources, Columbus, OH 43210 USA. [Lehmann, Johannes] Cornell Univ, Ithaca, NY 14853 USA. [O'Donnell, Anthony G.] Univ Western Australia, Fac Sci, Crawley, WA 6009, Australia. [Parton, William J.] Colorado State Univ, Nat Resource Ecol Lab, Ft Collins, CO 80523 USA. [Whitehead, David] New Zealand Landcare Res, New Zealand Agr Greenhouse Gas Res Ctr, Lincoln 7640, New Zealand. [Zimmermann, Michael] Univ Nat Resources & Life Sci Vienna, Dept Forest & Soil Sci, Inst Soil Res, A-1190 Vienna, Austria. RP Stockmann, U (reprint author), Univ Sydney, Fac Agr & Environm, Biomed Bldg C81,Suite 401,Cent Ave,Australian Tec, Eveleigh, NSW 2015, Australia. EM uta.stockmann@sydney.edu.au; mark.adams@sydney.edu.au; john.crawford@sydney.edu.au; damien.field@sydney.edu.au; mhen8672@uni.sydney.edu.au; meaghan.jenkins@sydney.edu.au; budiman.minasny@sydney.edu.au; Alex.McBratney@sydney.edu.au; vivien.deremydecourcelles@sydney.edu.au; kanika.singh@sydney.edu.au; ichsani.wheeler@sydney.edu.au; lynette.abbott@uwa.edu.au; denis.angers@agr.gc.ca; Jeff.Baldock@csiro.au; michael.bird@jcu.edu.au; philip.brookes@rothamsted.ac.uk; Claire.Chenu@grignon.inra.fr; jdjastrow@anl.gov; lal.1@osu.edu; CL273@cornell.edu; tony.odonnell@uwa.edu.au; billp@nrel.colostate.edu; WhiteheadD@landcareresearch.co.nz; michael.zimmermann@boku.ac.at RI adams, mark/H-1303-2012; Bird, Michael/G-5364-2010; Zimmermann, Michael/F-7547-2010; Lal, Rattan/D-2505-2013; James Cook University, TESS/B-8171-2012; Abbott, Lynette/F-7489-2011; McBratney, Alex/C-2199-2011; Lehmann, Johannes/H-2682-2014; Baldock, Jeffrey/G-1362-2010 OI Minasny, Budiman/0000-0002-1182-2371; Field, Damien/0000-0002-6877-8332; adams, mark/0000-0001-8989-508X; Bird, Michael/0000-0003-1801-8703; Jenkins, Meaghan/0000-0001-8403-4598; Zimmermann, Michael/0000-0002-5162-2008; Abbott, Lynette/0000-0001-8586-7858; Lehmann, Johannes/0000-0002-4701-2936; Baldock, Jeffrey/0000-0002-6428-8555 FU Dow Sustainability Program; ALCOA FX This review paper stems from the Soil Carbon Summit held in Sydney, Australia, in January 2011. The Summit was convened by the Soil Carbon Initiative, a project of the Dow Sustainability Program at the United States Studies Centre, in collaboration with the Faculty of Agriculture and Environment, both at The University of Sydney, Australia. The authors would like to acknowledge the financial support of this work by the Dow Sustainability Program and ALCOA. NR 180 TC 208 Z9 218 U1 66 U2 773 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-8809 EI 1873-2305 J9 AGR ECOSYST ENVIRON JI Agric. Ecosyst. Environ. PD JAN 1 PY 2013 VL 164 BP 80 EP 99 DI 10.1016/j.agee.2012.10.001 PG 20 WC Agriculture, Multidisciplinary; Ecology; Environmental Sciences SC Agriculture; Environmental Sciences & Ecology GA 097KM UT WOS:000315473000008 ER PT J AU Gilmanov, TG Wylie, BK Tieszen, LL Meyers, TP Baron, VS Bernacchi, CJ Billesbach, DP Burba, GG Fischer, ML Glenn, AJ Hanan, NP Hatfield, JL Heuer, MW Hollinger, SE Howard, DM Matamala, R Prueger, JH Tenuta, M Young, DG AF Gilmanov, Tagir G. Wylie, Bruce K. Tieszen, Larry L. Meyers, Tilden P. Baron, Vern S. Bernacchi, Carl J. Billesbach, David P. Burba, George G. Fischer, Marc L. Glenn, Aaron J. Hanan, Niall P. Hatfield, Jerry L. Heuer, Mark W. Hollinger, Steven E. Howard, Daniel M. Matamala, Roser Prueger, John H. Tenuta, Mario Young, David G. TI CO2 uptake and ecophysiological parameters of the grain crops of midcontinent North America: Estimates from flux tower measurements SO AGRICULTURE ECOSYSTEMS & ENVIRONMENT LA English DT Article DE Net CO2 exchange partitioning; Gross photosynthesis; VPD limitation of photosynthesis; CO2 sink; Maize; Wheat ID NET ECOSYSTEM EXCHANGE; GROSS PRIMARY PRODUCTION; CARBON-DIOXIDE EXCHANGE; LIGHT-RESPONSE PARAMETERS; NO-TILL ECOSYSTEM; UNITED-STATES; USE EFFICIENCY; EDDY COVARIANCE; PRIMARY PRODUCTIVITY; SURFACE-ENERGY AB We analyzed net CO2 exchange data from 13 flux tower sites with 27 site-years of measurements over maize and wheat fields across midcontinent North America. A numerically robust "light-soil temperature-VPD"-based method was used to partition the data into photosynthetic assimilation and ecosystem respiration components. Year-round ecosystem-scale ecophysiological parameters of apparent quantum yield, photosynthetic capacity, convexity of the light response, respiration rate parameters, ecological light-use efficiency, and the curvature of the VPD-response of photosynthesis for maize and wheat crops were numerically identified and interpolated/extrapolated. This allowed us to gap-fill CO2 exchange components and calculate annual totals and budgets. VPD-limitation of photosynthesis was systematically observed in grain crops of the region (occurring from 20 to 120 days during the growing season, depending on site and year), determined by the VPD regime and the numerical value of the curvature parameter of the photosynthesis-VPD-response, sigma(VPD). In 78% of the 27 site-years of observations, annual gross photosynthesis in these crops significantly exceeded ecosystem respiration, resulting in a net ecosystem production of up to 2100 g CO2 m(-2) year(-1). The measurement-based photosynthesis, respiration, and net ecosystem production data, as well as the estimates of the ecophysiological parameters, provide an empirical basis for parameterization and validation of mechanistic models of grain crop production in this economically and ecologically important region of North America. (C) 2012 Elsevier B.V. All rights reserved. C1 [Gilmanov, Tagir G.] S Dakota State Univ, Dept Nat Resource Management, Brookings, SD 57007 USA. [Wylie, Bruce K.; Tieszen, Larry L.] USGS EROS, Sioux Falls, SD 57198 USA. [Meyers, Tilden P.; Heuer, Mark W.] NOAA, Air Resources Lab, Atmospher Turbulence & Diffus Div, Oak Ridge, TN 37830 USA. [Baron, Vern S.] Lacombe Res Ctr, Lacombe, AB T4L 1W1, Canada. [Bernacchi, Carl J.] Univ Illinois, USDA ARS Photosynthesis Res Unit, Urbana, IL 61801 USA. [Bernacchi, Carl J.] Univ Illinois, Dept Plant Biol, Urbana, IL 61801 USA. [Billesbach, David P.] Univ Nebraska, Dept Biol Syst Engn, Lincoln, NE 68583 USA. [Burba, George G.] LI COR Biosci, Adv R&D, Lincoln, NE 68504 USA. [Fischer, Marc L.] Sustainable Energy Syst Grp, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Glenn, Aaron J.] Agr & Food Canada, Sci & Technol Branch, Brandon, MB R7A 5Y3, Canada. [Hanan, Niall P.] S Dakota State Univ, Geog Informat Sci Ctr, Brookings, SD 57007 USA. [Hatfield, Jerry L.] Natl Lab Agr & Environm, Ames, IA 50011 USA. [Heuer, Mark W.] Oak Ridge Associated Univ, Oak Ridge, TN 37830 USA. [Hollinger, Steven E.] Univ Illinois, Prairie Res Inst, Illinois State Water Survey, Ctr Atmospher Sci, Champaign, IL 61820 USA. [Howard, Daniel M.] US Geol Survey, Earth Resources Observat & Sci EROS Ctr, Sioux Falls, SD 57198 USA. [Matamala, Roser] Argonne Natl Lab, Biosci Div, Argonne, IL 60439 USA. [Prueger, John H.] Natl Lab Agr & Environm, Soil Water & Air Resources Res Unit, Ames, IA 50011 USA. [Tenuta, Mario] Univ Manitoba, Dept Soil Sci, Canada Res Chair Appl Soil Ecol, Winnipeg, MB R3T 2N2, Canada. [Young, David G.] Agr & Agri Food Canada, Crop & Soils Res Sect, Lacombe, AB T4L 1W1, Canada. RP Gilmanov, TG (reprint author), S Dakota State Univ, Dept Nat Resource Management, Brookings, SD 57007 USA. EM tagir.gilmanov@sdstate.edu; wylie@usgs.gov; llt@sio.midco.net; tilden.meyers@noaa.gov; vern.baron@agr.gc.ca; bernacch@illinois.edu; dbillesbach1@unl.edu; george.burba@licor.com; mlfischer@lbl.gov; aaron.glenn@agr.gc.ca; niall.hanan@sdstate.edu; jerry.hatfield@ars.usda.gov; mark.heuer@noaa.gov; hoboinc87@comcast.net; dhoward@usgs.gov; matamala@anl.gov; john.prueger@ars.usda.gov; mario.tenuta@ad.umanitoba.ca; david.young@agr.gc.ca RI Wylie, Bruce/H-3182-2014; Meyers, Tilden/C-6633-2016; Burba, George/G-9991-2014; OI Wylie, Bruce/0000-0002-7374-1083; Burba, George/0000-0003-2095-0057; Baron, Vern/0000-0001-5725-9230; Bernacchi, Carl/0000-0002-2397-425X; Howard, Daniel/0000-0002-7563-7538 FU USGS [G10PC00044]; USGS Geographic Analysis and Monitoring program; South Dakota Corn Utilization Council; Office of Biological and Environmental Research of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was performed under USGS contract G10PC00044 and funding was provided by the USGS Geographic Analysis and Monitoring program. This work was also supported in part by the grant from the South Dakota Corn Utilization Council. Measurements at the US-ARM site were supported by the Office of Biological and Environmental Research of the U.S. Department of Energy under contract DE-AC02-05CH11231 as part of the Atmospheric Radiation Measurement Program. We thank Ameriflux database supervisor Dr. Thomas Boden and Ameriflux contributors Drs. J. Baker, T. Griffis, A. Suyker, and S. Verma for assistance with the data needs of this project. NR 65 TC 15 Z9 16 U1 2 U2 66 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-8809 J9 AGR ECOSYST ENVIRON JI Agric. Ecosyst. Environ. PD JAN 1 PY 2013 VL 164 BP 162 EP 175 DI 10.1016/j.agee.2012.09.017 PG 14 WC Agriculture, Multidisciplinary; Ecology; Environmental Sciences SC Agriculture; Environmental Sciences & Ecology GA 097KM UT WOS:000315473000015 ER PT J AU de Boer, G Hashino, T Tripoli, GJ Eloranta, EW AF de Boer, G. Hashino, T. Tripoli, G. J. Eloranta, E. W. TI A numerical study of aerosol influence on mixed-phase stratiform clouds through modulation of the liquid phase SO ATMOSPHERIC CHEMISTRY AND PHYSICS LA English DT Article ID CENTRAL ARCTIC-OCEAN; ICE NUCLEATION; MARINE STRATOCUMULUS; CONDENSATION NUCLEI; IMMERSION MODE; PARTICLES; MICROPHYSICS; SENSITIVITY; SIMULATION; HEAT AB Numerical simulations were carried out in a high-resolution two-dimensional framework to increase our understanding of aerosol indirect effects in mixed-phase stratiform clouds. Aerosol characteristics explored include insoluble particle type, soluble mass fraction, influence of aerosol-induced freezing point depression and influence of aerosol number concentration. Simulations were analyzed with a focus on the processes related to liquid phase microphysics, and ice formation was limited to droplet freezing. Of the aerosol properties investigated, aerosol insoluble mass type and its associated freezing efficiency was found to be most relevant to cloud lifetime. Secondary effects from aerosol soluble mass fraction and number concentration also alter cloud characteristics and lifetime. These alterations occur via various mechanisms, including changes to the amount of nucleated ice, influence on liquid phase precipitation and ice riming rates, and changes to liquid droplet nucleation and growth rates. Alteration of the aerosol properties in simulations with identical initial and boundary conditions results in large variability in simulated cloud thickness and lifetime, ranging from rapid and complete glaciation of liquid to the production of long-lived, thick stratiform mixed-phase cloud. C1 [de Boer, G.] Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA. [de Boer, G.] NOAA, Earth Syst Res Lab, Div Phys Sci, Boulder, CO USA. [de Boer, G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Hashino, T.] Univ Tokyo, Atmosphere & Ocean Res Inst, Chiba, Japan. [Tripoli, G. J.; Eloranta, E. W.] Univ Wisconsin, Dept Atmospher & Ocean Sci, Madison, WI USA. RP de Boer, G (reprint author), Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA. EM gijs.deboer@colorado.edu RI de Boer, Gijs/F-3949-2011 OI de Boer, Gijs/0000-0003-4652-7150 FU Office of Science, Office of Biological and Environmental Research of the US Department of Energy [DE-AC02-05CH11231]; National Aeronautics and Space Administration [NASA: NNX07AQ81G]; United States Department of Energy [US DOE: DE-SC0008794]; NSF [ARC-1023366, ARC-1203902]; National Oceanic and Atmospheric Administration, US Department of Commerce [NA17RJ1229] FX The authors wish to acknowledge Dr. Karoline Diehl for her suggestions and assistance during the completion of this work and Hugh Morrison and Paquita Zuidema for their work in compiling the intercomparison document on which this work is based. Additionally, we'd like to thanks Drs. Matthew Shupe and David Turner for providing data for simulation validation. This research was supported in part by the Director, Office of Science, Office of Biological and Environmental Research of the US Department of Energy under Contract No. DE-AC02-05CH11231 as part of their Climate and Earth System Modeling Program, completed at the Lawrence Berkeley National Laboratory, managed by the University of California under the same grant. Finally, we would like to acknowledge additional funding from the National Aeronautics and Space Administration (NASA: NNX07AQ81G) and from the United States Department of Energy (US DOE: DE-SC0008794). G. B. was additionally supported by NSF grants ARC-1023366 and ARC-1203902. This work was prepared in part at the Cooperative Institute for Research in Environmental Sciences (CIRES) with support in part from the National Oceanic and Atmospheric Administration, US Department of Commerce, under cooperative agreement NA17RJ1229 and other grants. The statements, findings, conclusions, and recommendations are those of the author and do not necessarily reflect the views of the National Oceanic and Atmospheric Administration or the Department of Commerce. NR 50 TC 3 Z9 3 U1 0 U2 25 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1680-7316 J9 ATMOS CHEM PHYS JI Atmos. Chem. Phys. PY 2013 VL 13 IS 4 BP 1733 EP 1749 DI 10.5194/acp-13-1733-2013 PG 17 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 096LW UT WOS:000315406600003 ER PT J AU Yver, CE Graven, HD Lucas, DD Cameron-Smith, PJ Keeling, RF Weiss, RF AF Yver, C. E. Graven, H. D. Lucas, D. D. Cameron-Smith, P. J. Keeling, R. F. Weiss, R. F. TI Evaluating transport in the WRF model along the California coast SO ATMOSPHERIC CHEMISTRY AND PHYSICS LA English DT Article ID NONLOCAL CLOSURE-MODEL; ATMOSPHERIC BOUNDARY-LAYER; WEATHER RESEARCH; PART I; SCHEMES; PARAMETERIZATION; TURBULENCE; SYSTEM AB This paper presents a step in the development of a top-down method to complement the bottom-up inventories of halocarbon emissions in California using high frequency observations, forward simulations and inverse methods. The Scripps Institution of Oceanography high-frequency atmospheric halocarbons measurement sites are located along the California coast and therefore the evaluation of transport in the chosen Weather Research Forecast (WRF) model at these sites is crucial for inverse modeling. The performance of the transport model has been investigated by comparing the wind direction and speed and temperature at four locations using aircraft weather reports as well at all METAR weather stations in our domain for hourly variations. Different planetary boundary layer (PBL) schemes, horizontal resolutions (achieved through nesting) and two meteorological datasets have been tested. Finally, simulated concentration of an inert tracer has been briefly investigated. All the PBL schemes present similar results that generally agree with observations, except in summer when the model sea breeze is too strong. At the coarse 12 km resolution, using ERA-interim (ECMWF Re-Analysis) as initial and boundary conditions leads to improvements compared to using the North American Model (NAM) dataset. Adding higher resolution nests also improves the match with the observations. However, no further improvement is observed from increasing the nest resolution from 4 km to 0.8 km. Once optimized, the model is able to reproduce tracer measurements during typical winter California large-scale events (Santa Ana). Furthermore, with the WRF/CHEM chemistry module and the European Database for Global Atmospheric Research (EDGAR) version 4.1 emissions for HFC-134a, we find that using a simple emission scaling factor is not sufficient to infer emissions, which highlights the need for more complex inversions. C1 [Yver, C. E.; Graven, H. D.; Keeling, R. F.; Weiss, R. F.] Univ Calif San Diego, Scripps Inst Oceanog, La Jolla, CA 92093 USA. [Lucas, D. D.; Cameron-Smith, P. J.] Lawrence Livermore Natl Lab, Atmospher Earth & Energy Div, Livermore, CA 94550 USA. RP Yver, CE (reprint author), Univ Calif San Diego, Scripps Inst Oceanog, 9500 Gilman Dr, La Jolla, CA 92093 USA. EM cyver@ucsd.edu RI Cameron-Smith, Philip/E-2468-2011; OI Cameron-Smith, Philip/0000-0002-8802-8627; Graven, Heather/0000-0003-3934-2502 FU US National Institute of Science and Technology (NIST); US Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX Thanks to Wayne Angevine at NOAA, Anders Nottrott at UCSD, and the WRF support team for their advice on WRF configuration. We gratefully thank the WRF and Livermore Computing support teams. Super-computer resources were provided by Livermore Computing at the Lawrence Livermore National Laboratory. This work is funded by a grant from the US National Institute of Science and Technology (NIST). Part of this work was performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 34 TC 10 Z9 11 U1 0 U2 27 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1680-7316 J9 ATMOS CHEM PHYS JI Atmos. Chem. Phys. PY 2013 VL 13 IS 4 BP 1837 EP 1852 DI 10.5194/acp-13-1837-2013 PG 16 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 096LW UT WOS:000315406600009 ER PT J AU Myhre, G Samset, BH Schulz, M Balkanski, Y Bauer, S Berntsen, TK Bian, H Bellouin, N Chin, M Diehl, T Easter, RC Feichter, J Ghan, SJ Hauglustaine, D Iversen, T Kinne, S Kirkevag, A Lamarque, JF Lin, G Liu, X Lund, MT Luo, G Ma, X van Noije, T Penner, JE Rasch, PJ Ruiz, A Seland, O Skeie, RB Stier, P Takemura, T Tsigaridis, K Wang, P Wang, Z Xu, L Yu, H Yu, F Yoon, JH Zhang, K Zhang, H Zhou, C AF Myhre, G. Samset, B. H. Schulz, M. Balkanski, Y. Bauer, S. Berntsen, T. K. Bian, H. Bellouin, N. Chin, M. Diehl, T. Easter, R. C. Feichter, J. Ghan, S. J. Hauglustaine, D. Iversen, T. Kinne, S. Kirkevag, A. Lamarque, J. -F. Lin, G. Liu, X. Lund, M. T. Luo, G. Ma, X. van Noije, T. Penner, J. E. Rasch, P. J. Ruiz, A. Seland, O. Skeie, R. B. Stier, P. Takemura, T. Tsigaridis, K. Wang, P. Wang, Z. Xu, L. Yu, H. Yu, F. Yoon, J. -H. Zhang, K. Zhang, H. Zhou, C. TI Radiative forcing of the direct aerosol effect from AeroCom Phase II simulations SO ATMOSPHERIC CHEMISTRY AND PHYSICS LA English DT Article ID SECONDARY ORGANIC AEROSOL; ENERGY SYSTEM CERES; GLOBAL-MODEL; BLACK CARBON; ANTHROPOGENIC INFLUENCE; PREINDUSTRIAL TIMES; RELATIVE-HUMIDITY; OPTICAL-THICKNESS; LIGHT-ABSORPTION; DUST AEROSOLS AB We report on the AeroCom Phase II direct aerosol effect (DAE) experiment where 16 detailed global aerosol models have been used to simulate the changes in the aerosol distribution over the industrial era. All 16 models have estimated the radiative forcing (RF) of the anthropogenic DAE, and have taken into account anthropogenic sulphate, black carbon (BC) and organic aerosols (OA) from fossil fuel, biofuel, and biomass burning emissions. In addition several models have simulated the DAE of anthropogenic nitrate and anthropogenic influenced secondary organic aerosols (SOA). The model simulated all-sky RF of the DAE from total anthropogenic aerosols has a range from -0.58 to -0.02 Wm(-2), with a mean of -0.27 Wm(-2) for the 16 models. Several models did not include nitrate or SOA and modifying the estimate by accounting for this with information from the other AeroCom models reduces the range and slightly strengthens the mean. Modifying the model estimates for missing aerosol components and for the time period 1750 to 2010 results in a mean RF for the DAE of -0.35 Wm(-2). Compared to AeroCom Phase I (Schulz et al., 2006) we find very similar spreads in both total DAE and aerosol component RF. However, the RF of the total DAE is stronger negative and RF from BC from fossil fuel and biofuel emissions are stronger positive in the present study than in the previous AeroCom study. We find a tendency for models having a strong (positive) BC RF to also have strong (negative) sulphate or OA RF. This relationship leads to smaller uncertainty in the total RF of the DAE compared to the RF of the sum of the individual aerosol components. The spread in results for the individual aerosol components is substantial, and can be divided into diversities in burden, mass extinction coefficient (MEC), and normalized RF with respect to AOD. We find that these three factors give similar contributions to the spread in results. C1 [Myhre, G.; Samset, B. H.; Berntsen, T. K.; Lund, M. T.; Skeie, R. B.] CICERO, Oslo, Norway. [Schulz, M.; Iversen, T.; Kirkevag, A.; Seland, O.] Norwegian Meteorol Inst, Oslo, Norway. [Balkanski, Y.; Hauglustaine, D.] CEA CNRS UVSQ, Lab Sci Climat & Environm, Gif Sur Yvette, France. [Bauer, S.] NASA, Goddard Inst Space Studies, New York, NY 10025 USA. [Bauer, S.; Tsigaridis, K.] Columbia Earth Inst, New York, NY USA. [Bian, H.; Yu, H.] Univ Maryland, Earth Syst Sci Interdisciplinary Ctr, College Pk, MD 20742 USA. [Bellouin, N.] Met Off Hadley Ctr, Exeter, Devon, England. [Chin, M.; Diehl, T.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Diehl, T.; Liu, X.] Univ Space Res Assoc, Columbia, MD USA. [Easter, R. C.; Ghan, S. J.; Rasch, P. J.; Yoon, J. -H.; Zhang, K.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Feichter, J.; Kinne, S.; Zhang, K.] Max Planck Inst Meteorol, D-20146 Hamburg, Germany. [Iversen, T.] Univ Oslo, Dept Geosci, Oslo, Norway. [Lamarque, J. -F.] Natl Ctr Atmospher Res, NCAR Earth Syst Lab, Boulder, CO 80307 USA. [Lin, G.; Penner, J. E.; Xu, L.; Zhou, C.] Univ Michigan, Dept Atmospher Ocean & Space Sci, Ann Arbor, MI 48109 USA. [Luo, G.; Ma, X.; Yu, F.] SUNY Albany, Atmospher Sci Res Ctr, Albany, NY 12222 USA. [van Noije, T.; Ruiz, A.; Wang, P.] Royal Netherlands Meteorol Inst, NL-3730 AE De Bilt, Netherlands. [Ruiz, A.] Univ Zaragoza, CSIC, LIFTEC, Zaragoza, Spain. [Stier, P.] Univ Oxford, Dept Phys, Oxford, England. [Takemura, T.] Kyushu Univ, Appl Mech Res Inst, Fukuoka 8168580, Japan. [Wang, Z.] Chinese Acad Meteorol Sci, Beijing 100081, Peoples R China. [Xu, L.] Univ Calif San Diego, Scripps Inst Oceanog, La Jolla, CA 92093 USA. [Zhang, H.] China Meteorol Adm, Natl Climate Ctr, Lab Climate Studies, Beijing 100081, Peoples R China. RP Myhre, G (reprint author), CICERO, Oslo, Norway. EM gunnar.myhre@cicero.uio.no RI Kyushu, RIAM/F-4018-2015; Yu, Hongbin/C-6485-2008; Takemura, Toshihiko/C-2822-2009; Penner, Joyce/J-1719-2012; Chin, Mian/J-8354-2012; ma, xiaoyan/D-2308-2014; YOON, JIN-HO/A-1672-2009; Liu, Xiaohong/E-9304-2011; Yu, Fangqun/F-3708-2011; Balkanski, Yves/A-6616-2011; Lamarque, Jean-Francois/L-2313-2014; Bauer, Susanne/P-3082-2014; Myhre, Gunnar/A-3598-2008; Zhang, Kai/F-8415-2010; Skeie, Ragnhild/K-1173-2015; Schulz, Michael/A-6930-2011; U-ID, Kyushu/C-5291-2016; Ghan, Steven/H-4301-2011; Lund, Marianne /J-6465-2016; Stier, Philip/B-2258-2008 OI Zhou, Cheng/0000-0001-9095-2846; Yu, Hongbin/0000-0003-4706-1575; Takemura, Toshihiko/0000-0002-2859-6067; YOON, JIN-HO/0000-0002-4939-8078; Liu, Xiaohong/0000-0002-3994-5955; Yu, Fangqun/0000-0003-0874-4883; Balkanski, Yves/0000-0001-8241-2858; Lamarque, Jean-Francois/0000-0002-4225-5074; Myhre, Gunnar/0000-0002-4309-476X; Zhang, Kai/0000-0003-0457-6368; Skeie, Ragnhild/0000-0003-1246-4446; Schulz, Michael/0000-0003-4493-4158; Ghan, Steven/0000-0001-8355-8699; Lund, Marianne /0000-0001-9911-4160; Stier, Philip/0000-0002-1191-0128 FU US Department of Energy, Office of Science, Scientific Discovery through Advanced Computing (SciDAC) Program; Office of Science Earth System Modeling Program; National Science Foundation; DOE by Battelle Memorial Institute [DE-AC06- 76RLO 1830]; FP6 project EUCAARI [34684]; Research Council of Norway through the EarthClim project [207711/E10]; Research Council of Norway through the NOTUR/NorStore project; Norwegian Space Centre through PM-VRAE; EU project PEGASOS; EU project ACCESS; National Basic Research Program of China [2011CB403405]; US NSF [AGS-0942106]; NASA [NNX11AQ72G]; NASA-MAP [NNX09AK32G]; Joint DECC/Defra Met Office Hadley Centre Climate Programme [GA01101]; Research Council of Norway through the SLAC project; EU-project ECLIPSE FX S. Ghan, X. Liu, R. Easter, P. Rasch and J.-H. Yoon were funded by the US Department of Energy, Office of Science, Scientific Discovery through Advanced Computing (SciDAC) Program and by the Office of Science Earth System Modeling Program. Computing resources were provided by the Climate Simulation Laboratory at NCAR's Computational and Information Systems Laboratory (CISL), sponsored by the National Science Foundation and other agencies. The Pacific Northwest National Laboratory is operated for DOE by Battelle Memorial Institute under contract DE-AC06- 76RLO 1830. Simulations of the ECHAM5-HAM, INCA, CAM4-Oslo and HadGEM2 models have been supported with funds from the FP6 project EUCAARI (Contract 34684). A. Kirkevag, T. Iversen and O. Seland (CAM4-Oslo) were supported by the Research Council of Norway through the EarthClim (207711/E10) and NOTUR/NorStore projects, by the Norwegian Space Centre through PM-VRAE, and through the EU projects PEGASOS and ACCESS. H. Zhang and Z. Wang were funded by National Basic Research Program of China (2011CB403405). G. Luo, X. Ma and F. Yu were funded by the US NSF (AGS-0942106) and NASA (NNX11AQ72G). K. Tsigaridis and S. Bauer were supported by NASA-MAP (NASA award NNX09AK32G). Resources supporting this work were provided by the NASA High-End Computing (HEC) Program through the NASA Center for Climate Simulation (NCCS) at Goddard Space Flight Center. N. Bellouin was supported by the Joint DECC/Defra Met Office Hadley Centre Climate Programme (GA01101). G. Myhre and B. Samset were funded by the Research Council of Norway through the EarthClim and SLAC projects and the EU-project ECLIPSE. NR 94 TC 180 Z9 183 U1 19 U2 149 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1680-7316 EI 1680-7324 J9 ATMOS CHEM PHYS JI Atmos. Chem. Phys. PY 2013 VL 13 IS 4 BP 1853 EP 1877 DI 10.5194/acp-13-1853-2013 PG 25 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 096LW UT WOS:000315406600010 ER PT J AU Kalenderski, S Stenchikov, G Zhao, C AF Kalenderski, S. Stenchikov, G. Zhao, C. TI Modeling a typical winter-time dust event over the Arabian Peninsula and the Red Sea SO ATMOSPHERIC CHEMISTRY AND PHYSICS LA English DT Article ID AEROSOL OPTICAL-PROPERTIES; SKY RADIANCE MEASUREMENTS; MINERAL DUST; SAHARAN DUST; WEST-AFRICA; SYSTEM; OCEAN; VARIABILITY; TRANSPORT; SURFACE AB We used WRF-Chem, a regional meteorological model coupled with an aerosol-chemistry component, to simulate various aspects of the dust phenomena over the Arabian Peninsula and Red Sea during a typical winter-time dust event that occurred in January 2009. The model predicted that the total amount of emitted dust was 18.3 Tg for the entire dust outburst period and that the two maximum daily rates were similar to 2.4 Tg day(-1) and similar to 1.5 Tg day(-1), corresponding to two periods with the highest aerosol optical depth that were well captured by ground-and satellite-based observations. The model predicted that the dust plume was thick, extensive, and mixed in a deep boundary layer at an altitude of 3-4 km. Its spatial distribution was modeled to be consistent with typical spatial patterns of dust emissions. We utilized MODIS-Aqua and Solar Village AERONET measurements of the aerosol optical depth (AOD) to evaluate the radiative impact of aerosols. Our results clearly indicated that the presence of dust particles in the atmosphere caused a significant reduction in the amount of solar radiation reaching the surface during the dust event. We also found that dust aerosols have significant impact on the energy and nutrient balances of the Red Sea. Our results showed that the simulated cooling under the dust plume reached 100 W m(-2), which could have profound effects on both the sea surface temperature and circulation. Further analysis of dust generation and its spatial and temporal variability is extremely important for future projections and for better understanding of the climate and ecological history of the Red Sea. C1 [Kalenderski, S.; Stenchikov, G.] King Abdullah Univ Sci & Technol, Div Phys Sci & Engn, Thuwal, Saudi Arabia. [Zhao, C.] Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. RP Kalenderski, S (reprint author), King Abdullah Univ Sci & Technol, Div Phys Sci & Engn, Thuwal, Saudi Arabia. EM stoitchko.kalenderski@kaust.edu.sa RI Zhao, Chun/A-2581-2012; Georgiy, Stenchikov/J-8569-2013; OI Zhao, Chun/0000-0003-4693-7213; Stenchikov, Georgiy Lvovich/0000-0001-9033-4925 FU King Abdullah University of Science and Technology; US Department of Energy FX Stoitchko Kalenderski was partially supported by the King Abdullah University of Science and Technology Academic Excellence Alliance grant "Dust Storms and Climate Change". C. Zhao was partially supported by the Earth System Modeling Program of the US Department of Energy in scope of the project "Investigations on the Magnitude and Probabilities of Abrupt Climate Transitions". We thank Martin Dameris for the editorial guidance. The insightful comments offered by Sebastian Otto and both anonymous referees are highly appreciated. NR 73 TC 20 Z9 20 U1 0 U2 23 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1680-7316 J9 ATMOS CHEM PHYS JI Atmos. Chem. Phys. PY 2013 VL 13 IS 4 BP 1999 EP 2014 DI 10.5194/acp-13-1999-2013 PG 16 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 096LW UT WOS:000315406600018 ER PT J AU Young, PJ Archibald, AT Bowman, KW Lamarque, JF Naik, V Stevenson, DS Tilmes, S Voulgarakis, A Wild, O Bergmann, D Cameron-Smith, P Cionni, I Collins, WJ Dalsoren, SB Doherty, RM Eyring, V Faluvegi, G Horowitz, LW Josse, B Lee, YH MacKenzie, IA Nagashima, T Plummer, DA Righi, M Rumbold, ST Skeie, RB Shindell, DT Strode, SA Sudo, K Szopa, S Zeng, G AF Young, P. J. Archibald, A. T. Bowman, K. W. Lamarque, J. -F. Naik, V. Stevenson, D. S. Tilmes, S. Voulgarakis, A. Wild, O. Bergmann, D. Cameron-Smith, P. Cionni, I. Collins, W. J. Dalsoren, S. B. Doherty, R. M. Eyring, V. Faluvegi, G. Horowitz, L. W. Josse, B. Lee, Y. H. MacKenzie, I. A. Nagashima, T. Plummer, D. A. Righi, M. Rumbold, S. T. Skeie, R. B. Shindell, D. T. Strode, S. A. Sudo, K. Szopa, S. Zeng, G. TI Pre-industrial to end 21st century projections of tropospheric ozone from the Atmospheric Chemistry and Climate Model Intercomparison Project (ACCMIP) SO ATMOSPHERIC CHEMISTRY AND PHYSICS LA English DT Article ID GLOBAL LIGHTNING DISTRIBUTIONS; NORTH-ATLANTIC OSCILLATION; METHANE EMISSION CONTROLS; AIR-POLLUTION TRANSPORT; ISOPRENE EMISSIONS; SURFACE OZONE; STRATOSPHERIC OZONE; MULTIMODEL ASSESSMENT; TROPOPAUSE HEIGHT; FUTURE CHANGES AB Present day tropospheric ozone and its changes between 1850 and 2100 are considered, analysing 15 global models that participated in the Atmospheric Chemistry and Climate Model Intercomparison Project (ACCMIP). The ensemble mean compares well against present day observations. The seasonal cycle correlates well, except for some locations in the tropical upper troposphere. Most (75%) of the models are encompassed with a range of global mean tropospheric ozone column estimates from satellite data, but there is a suggestion of a high bias in the Northern Hemisphere and a low bias in the Southern Hemisphere, which could indicate deficiencies with the ozone precursor emissions. Compared to the present day ensemble mean tropospheric ozone burden of 337 +/- 23 Tg, the ensemble mean burden for 1850 time slice is similar to 30% lower. Future changes were modelled using emissions and climate projections from four Representative Concentration Pathways (RCPs). Compared to 2000, the relative changes in the ensemble mean tropospheric ozone burden in 2030 (2100) for the different RCPs are: -4% (-16%) for RCP2.6, 2% (-7%) for RCP4.5, 1% (-9%) for RCP6.0, and 7% (18%) for RCP8.5. Model agreement on the magnitude of the change is greatest for larger changes. Reductions in most precursor emissions are common across the RCPs and drive ozone decreases in all but RCP8.5, where doubled methane and a 40-150% greater stratospheric influx (estimated from a subset of models) increase ozone. While models with a high ozone burden for the present day also have high ozone burdens for the other time slices, no model consistently predicts large or small ozone changes; i.e. the magnitudes of the burdens and burden changes do not appear to be related simply, and the models are sensitive to emissions and climate changes in different ways. Spatial patterns of ozone changes are well correlated across most models, but are notably different for models without time evolving stratospheric ozone concentrations. A unified approach to ozone budget specifications and a rigorous investigation of the factors that drive tropospheric ozone is recommended to help future studies attribute ozone changes and inter-model differences more clearly. C1 [Young, P. J.] Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA. [Young, P. J.] NOAA, Div Chem Sci, Earth Syst Res Lab, Boulder, CO USA. [Archibald, A. T.] Univ Cambridge, Ctr Atmospher Sci, Cambridge, England. [Archibald, A. T.] Univ Cambridge, Natl Ctr Atmospher Sci, Cambridge, England. [Bowman, K. W.] NASA, Jet Prop Lab, Pasadena, CA USA. [Lamarque, J. -F.; Tilmes, S.] Natl Ctr Atmospher Res, Boulder, CO 80307 USA. [Naik, V.] NOAA, UCAR, Geophys Fluid Dynam Lab, Princeton, NJ USA. [Stevenson, D. S.; Doherty, R. M.; MacKenzie, I. A.] Univ Edinburgh, Sch GeoSci, Edinburgh, Midlothian, Scotland. [Voulgarakis, A.] Univ London Imperial Coll Sci Technol & Med, Dept Phys, London, England. [Young, P. J.; Wild, O.] Univ Lancaster, Lancaster Environm Ctr, Lancaster, England. [Bergmann, D.; Cameron-Smith, P.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Cionni, I.] Agenzia Nazl Nuove Tecnol Energia & Sviluppo Econ, Bologna, Italy. [Collins, W. J.; Rumbold, S. T.] Met Off Hadley Ctr, Exeter, Devon, England. [Dalsoren, S. B.; Skeie, R. B.] Ctr Int Climate & Environm Res Oslo, Oslo, Norway. [Eyring, V.; Righi, M.] Deutsch Zentrum Luft & Raumfahrt DLR, Inst Phys Atmosphare, Oberpfaffenhofen, Germany. [Faluvegi, G.; Lee, Y. H.; Shindell, D. T.] NASA, Goddard Inst Space Studies, New York, NY 10025 USA. [Faluvegi, G.; Lee, Y. H.; Shindell, D. T.] Columbia Univ, Columbia Earth Inst, New York, NY USA. [Horowitz, L. W.] NOAA, Geophys Fluid Dynam Lab, Princeton, NJ USA. [Josse, B.] Ctr Natl Rech Meteorol, CNRS, GAME CNRM, Toulouse, France. [Nagashima, T.] Japan Marine Sci & Technol Ctr, Frontier Res Ctr Global Change, Yokohama, Kanagawa, Japan. [Plummer, D. A.] Environm Canada, Canadian Ctr Climate Modeling & Anal, Victoria, BC, Canada. [Strode, S. A.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Strode, S. A.] Univ Space Res Assoc, Columbia, MD USA. [Sudo, K.] Nagoya Univ, Grad Sch Environm Studies, Dept Earth & Environm Sci, Nagoya, Aichi 4648601, Japan. [Szopa, S.] LSCE CEA CNRS UVSQ, Lab Sci Climat & Environm, Gif Sur Yvette, France. [Zeng, G.] Natl Inst Water & Atmospher Res, Lauder, New Zealand. RP Young, PJ (reprint author), Univ Lancaster, Lancaster Environm Ctr, Lancaster, England. EM paul.j.young@lancaster.ac.uk RI Skeie, Ragnhild/K-1173-2015; Strode, Sarah/H-2248-2012; Eyring, Veronika/O-9999-2016; Lee, Yunha/Q-7222-2016; Manager, CSD Publications/B-2789-2015; Wild, Oliver/A-4909-2009; Collins, William/A-5895-2010; mackenzie, ian/E-9320-2013; Bergmann, Daniel/F-9801-2011; Righi, Mattia/I-5120-2013; Cameron-Smith, Philip/E-2468-2011; Szopa, Sophie/F-8984-2010; Shindell, Drew/D-4636-2012; Horowitz, Larry/D-8048-2014; Naik, Vaishali/A-4938-2013; Lamarque, Jean-Francois/L-2313-2014; Young, Paul/E-8739-2010; Stevenson, David/C-8089-2012 OI Skeie, Ragnhild/0000-0003-1246-4446; Strode, Sarah/0000-0002-8103-1663; Eyring, Veronika/0000-0002-6887-4885; Lee, Yunha/0000-0001-7478-2672; Righi, Mattia/0000-0003-3827-5950; Wild, Oliver/0000-0002-6227-7035; Collins, William/0000-0002-7419-0850; Bergmann, Daniel/0000-0003-4357-6301; Cameron-Smith, Philip/0000-0002-8802-8627; Szopa, Sophie/0000-0002-8641-1737; Horowitz, Larry/0000-0002-5886-3314; Naik, Vaishali/0000-0002-2254-1700; Lamarque, Jean-Francois/0000-0002-4225-5074; Young, Paul/0000-0002-5608-8887; Stevenson, David/0000-0002-4745-5673 FU International Global Atmospheric Chemistry (IGAC); Stratospheric Processes And their Role in Climate (SPARC) projects; US Dept. of Energy (BER); LLNL [DE-AC52-07NA27344]; NERSC [DE-AC02-05CH11231]; Norwegian Research Council; DLR Earth System Model Validation (ESMVal) project; ENEA National Integrated Model; NASA Modeling, Analysis and Prediction program; DECC [GA01101]; Defra Integrated Climate Programme [GA01101]; Ministry of the Environment, Japan [S-7]; National Science Foundation; Office of Science (BER) of the US Department of Energy; UK research council [NE/I008063/1]; New Zealand Ministry of Science and Innovation FX ACCMIP is organised under the auspices of the International Global Atmospheric Chemistry (IGAC) and Stratospheric Processes And their Role in Climate (SPARC) projects, which fall under the International Geosphere-Biosphere Project (IGBP) and World Climate Research Program (WCRP) respectively. The authors are grateful to the British Atmospheric Data Centre (BADC), which is part of the NERC National Centre for Atmospheric Science (NCAS), for collecting and archiving the ACCMIP data. For CESM-CAM-superfast, DB and PC were funded by the US Dept. of Energy (BER) and simulations were performed under the auspices of LLNL under Contract DE-AC52-07NA27344, and using the supercomputing resources of NERSC under contract No. DE-AC02-05CH11231. The CICERO-OsloCTM2 simulations were completed within the projects SLAC (Short Lived Atmospheric Components) and EarthClim funded by the Norwegian Research Council. DP would like to thank the Canadian Foundation for Climate and Atmospheric Sciences for their long-running support of CMAM development. For EMAC, the work of VE and MR was funded by the DLR Earth System Model Validation (ESMVal) project and used the supercomputing resources of the German Climate Computing Center (DKRZ) and the Leibniz Supercomputing Centre (LRZ), and the work of IC was funded by the ENEA National Integrated Model to support the international negotiation on atmospheric pollution (Minni) project. The GEOSCCM work was supported by the NASA Modeling, Analysis and Prediction program, with computing resources provided by NASA's High-End Computing Program through the NASA Advanced Supercomputing Division. VN and LWH acknowledge efforts of GFDL's Global Atmospheric Model Development Team in the development of the GFDL-AM3 and Modeling Services Group for assistance with data processing. For the GISS models, support is acknowledged from the NASA MAP and ACMAP programs. For HadGEM2, WJC and STR were supported by the Joint DECC and Defra Integrated Climate Programme (GA01101). The LMDz-OR-INCA simulations were done using computing resources provided by the CCRT/GENCI computer centre of the CEA. The MOCAGE simulations were supported by Meteo-France and CNRS and supercomputing time was provided by the Meteo-France/DSI supercomputing centre. The MIROC-CHEM calculations were performed on the NIES supercomputer system (NEC SX-8R), and supported by the Environment Research and Technology Development Fund (S-7) of the Ministry of the Environment, Japan. The CESM project, including NCAR-CAM3.5, is supported by the National Science Foundation and the Office of Science (BER) of the US Department of Energy. The National Center for Atmospheric Research is operated by the University Corporation for Atmospheric Research under sponsorship of the National Science Foundation. The STOC-HadAM3 work was supported by cross UK research council grant NE/I008063/1 and used facilities provided by the UK's national high-performance computing service, HECToR, through Computational Modelling Services (CMS), part of the NERC National Centre for Atmospheric Science (NCAS). For UM-CAM, GZ acknowledges NIWA HPCF facility and funding from New Zealand Ministry of Science and Innovation. NR 121 TC 130 Z9 135 U1 7 U2 125 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1680-7316 EI 1680-7324 J9 ATMOS CHEM PHYS JI Atmos. Chem. Phys. PY 2013 VL 13 IS 4 BP 2063 EP 2090 DI 10.5194/acp-13-2063-2013 PG 28 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 096LW UT WOS:000315406600022 ER PT J AU Shilling, JE Zaveri, RA Fast, JD Kleinman, L Alexander, ML Canagaratna, MR Fortner, E Hubbe, JM Jayne, JT Sedlacek, A Setyan, A Springston, S Worsnop, DR Zhang, Q AF Shilling, J. E. Zaveri, R. A. Fast, J. D. Kleinman, L. Alexander, M. L. Canagaratna, M. R. Fortner, E. Hubbe, J. M. Jayne, J. T. Sedlacek, A. Setyan, A. Springston, S. Worsnop, D. R. Zhang, Q. TI Enhanced SOA formation from mixed anthropogenic and biogenic emissions during the CARES campaign SO ATMOSPHERIC CHEMISTRY AND PHYSICS LA English DT Article ID SECONDARY ORGANIC AEROSOL; REACTION MASS-SPECTROMETER; HIGH-RESOLUTION; PTR-MS; CARBONACEOUS AEROSOL; SUBMICRON PARTICLES; ELEMENTAL ANALYSIS; TROPICAL FOREST; MEXICO-CITY; ISOPRENE AB The CARES campaign was conducted during June, 2010 in the vicinity of Sacramento, California to study aerosol formation and aging in a region where anthropogenic and biogenic emissions regularly mix. Here, we describe measurements from an Aerodyne High Resolution Aerosol Mass Spectrometer (AMS), an Ionicon Proton Transfer Reaction Mass Spectrometer (PTR-MS), and trace gas detectors (CO, NO, NOx) deployed on the G-1 research aircraft to investigate ambient gas-and particle-phase chemical composition. AMS measurements showed that the particle phase is dominated by organic aerosol (OA) (85% on average) with smaller concentrations of sulfate (5%), nitrate (6%) and ammonium (3%) observed. PTR-MS data showed that isoprene dominated the biogenic volatile organic compound concentrations (BVOCs), with monoterpene concentrations generally below the detection limit. Using two different metrics, median OA concentrations and the slope of plots of OA vs. CO concentrations (i.e. Delta OA/Delta CO), we contrast organic aerosol evolution on flight days with different prevailing meteorological conditions to elucidate the role of anthropogenic and biogenic emissions on OA formation. Airmasses influenced predominantly by biogenic emissions had median OA concentrations of 2.2 mu g m(-3) and near zero Delta OA/Delta CO. Those influenced predominantly by anthropogenic emissions had median OA concentrations of 4.7 mu g m(-3) and Delta OA/Delta CO ratios of 35-44 mu g m(-3) ppmv. But, when biogenic and anthropogenic emissions mixed, OA levels were enhanced, with median OA concentrations of 11.4 mu g m(-3) and Delta OA/Delta CO ratios of 77-157 mu g m(-3) ppmv. Taken together, our observations show that production of OA was enhanced when anthropogenic emissions from Sacramento mixed with isoprene-rich air from the foothills. After considering several anthropogenic/biogenic interaction mechanisms, we conclude that NOx concentrations play a strong role in enhancing SOA formation from isoprene, though the chemical mechanism for the enhancement remains unclear. If these observations are found to be robust in other seasons and in areas outside of Sacramento, regional and global aerosol modules will need to incorporate more complex representations of NOx-dependent SOA mechanisms and yields into their algorithms. Ultimately, accurately predicting OA mass concentrations and their effect on radiation balance will require a mechanistically-based treatment of the interactions of biogenic and anthropogenic emissions. C1 [Shilling, J. E.; Zaveri, R. A.; Fast, J. D.; Hubbe, J. M.] Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. [Kleinman, L.; Sedlacek, A.; Springston, S.] Brookhaven Natl Lab, Div Atmospher Sci, Upton, NY 11973 USA. [Alexander, M. L.] Pacific NW Natl Lab, Environm & Mol Sci Lab, Richland, WA 99352 USA. [Canagaratna, M. R.; Fortner, E.; Jayne, J. T.; Worsnop, D. R.] Aerodyne Res Inc, Billerica, MA 01821 USA. [Setyan, A.; Zhang, Q.] Univ Calif Davis, Dept Environm Toxicol, Davis, CA 95616 USA. RP Shilling, JE (reprint author), Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. EM john.shilling@pnnl.gov RI Shilling, John/L-6998-2015; Setyan, Ari/C-4025-2011; Zhang, Qi/F-9653-2010; Worsnop, Douglas/D-2817-2009 OI Shilling, John/0000-0002-3728-0195; Zaveri, Rahul/0000-0001-9874-8807; Setyan, Ari/0000-0002-9078-6478; Worsnop, Douglas/0000-0002-8928-8017 FU Atmospheric Radiation Measurement (ARM) Climate Research Facility; U.S. Department of Energy (DOE), Office of Biological and Environmental Research (OBER); Environmental Molecular Sciences Laboratory (EMSL); DOE's OBER at Pacific Northwest National Laboratory (PNNL); US DOE's Atmospheric System Research Program at PNNL [DE-AC06-76RLO 1830] FX The authors thank the G-1 flight and ground crews for supporting the CARES mission. Funding for data collection onboard the G-1 aircraft and at the ground sites was provided by the Atmospheric Radiation Measurement (ARM) Climate Research Facility sponsored by the U.S. Department of Energy (DOE), Office of Biological and Environmental Research (OBER). Partial support was also provided by the Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by the DOE's OBER at Pacific Northwest National Laboratory (PNNL). Data analysis and research was supported by the US DOE's Atmospheric System Research Program under Contract DE-AC06-76RLO 1830 at PNNL. PNNL is operated for the US DOE by Battelle Memorial Institute. NR 67 TC 42 Z9 42 U1 6 U2 123 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1680-7316 EI 1680-7324 J9 ATMOS CHEM PHYS JI Atmos. Chem. Phys. PY 2013 VL 13 IS 4 BP 2091 EP 2113 DI 10.5194/acp-13-2091-2013 PG 23 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 096LW UT WOS:000315406600023 ER PT J AU He, P Wei, B Wang, S Stock, SR Yu, HY Wang, G AF He, Peng Wei, Biao Wang, Steve Stock, Stuart R. Yu, Hengyong Wang, Ge TI Piecewise-Constant-Model-Based Interior Tomography Applied to Dentin Tubules SO COMPUTATIONAL AND MATHEMATICAL METHODS IN MEDICINE LA English DT Article ID ITERATIVE ALGORITHMS; IMAGE-RECONSTRUCTION; PROJECTION DATA; HUMAN TEETH; RAY; MICROSCOPY; SART; ART AB Dentin is a hierarchically structured biomineralized composite material, and dentin's tubules are difficult to study in situ. Nano-CT provides the requisite resolution, but the field of view typically contains only a few tubules. Using a plate-like specimen allows reconstruction of a volume containing specific tubules from a number of truncated projections typically collected over an angular range of about 140 degrees, which is practically accessible. Classical computed tomography (CT) theory cannot exactly reconstruct an object only from truncated projections, needless to say a limited angular range. Recently, interior tomography was developed to reconstruct a region-of-interest (ROI) from truncated data in a theoretically exact fashion via the total variation (TV) minimization under the condition that the ROI is piecewise constant. In this paper, we employ a TV minimization interior tomography algorithm to reconstruct interior microstructures in dentin from truncated projections over a limited angular range. Compared to the filtered backprojection (FBP) reconstruction, our reconstruction method reduces noise and suppresses artifacts. Volume rendering confirms the merits of our method in terms of preserving the interior microstructure of the dentin specimen. C1 [He, Peng; Wei, Biao] Chongqing Univ, Educ Minist China, Key Lab Optoelect Technol & Syst, Chongqing 400044, Peoples R China. [He, Peng; Yu, Hengyong; Wang, Ge] Virginia Tech, VT WFU Sch Biomed Engn & Sci, Biomed Imaging Div, Blacksburg, VA 24061 USA. [Wang, Steve] Argonne Natl Lab, Argonne, IL 60439 USA. [Stock, Stuart R.] Northwestern Univ, Feinberg Sch Med, Dept Mol Pharmacol & Biol Chem, Chicago, IL 60611 USA. [Yu, Hengyong; Wang, Ge] Wake Forest Univ Hlth Sci, VT WFU Sch Biomed Engn & Sci, Biomed Imaging Div, Winston Salem, NC 27157 USA. RP Wei, B (reprint author), Chongqing Univ, Educ Minist China, Key Lab Optoelect Technol & Syst, Chongqing 400044, Peoples R China. EM weibiao@cqu.edu.cn; ge-wang@ieee.org FU US NIH/NIBIB [EB011785]; US NICDR [DE001374]; National Natural Science Foundation of China [61171157]; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work was partially supported by the US NIH/NIBIB Grant EB011785, US NICDR Grant DE001374, and the National Natural Science Foundation of China Grant 61171157. The use of the Advanced Photon Source was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract no. DE-AC02-06CH11357. NR 28 TC 2 Z9 2 U1 1 U2 9 PU HINDAWI PUBLISHING CORPORATION PI NEW YORK PA 410 PARK AVENUE, 15TH FLOOR, #287 PMB, NEW YORK, NY 10022 USA SN 1748-670X EI 1748-6718 J9 COMPUT MATH METHOD M JI Comput. Math. Method Med. PY 2013 AR 892451 DI 10.1155/2013/892451 PG 8 WC Mathematical & Computational Biology SC Mathematical & Computational Biology GA 098EH UT WOS:000315528800001 ER PT J AU Datta, MK Kadakia, K Velikokhatnyi, OI Jampani, PH Chung, SJ Poston, JA Manivannan, A Kumta, PN AF Datta, Moni Kanchan Kadakia, Karan Velikokhatnyi, Oleg I. Jampani, Prashanth H. Chung, Sung Jae Poston, James A. Manivannan, Ayyakkannu Kumta, Prashant N. TI High performance robust F-doped tin oxide based oxygen evolution electro-catalysts for PEM based water electrolysis SO JOURNAL OF MATERIALS CHEMISTRY A LA English DT Article ID TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; HYDROGEN ENERGY; SULFURIC-ACID; ELECTROCATALYSTS; FILMS; PHOSPHATE; EFFICIENT; BEHAVIOR AB Identification and development of non-noble metal based electro-catalysts or electro-catalysts comprising compositions with significantly reduced amounts of expensive noble metal contents (e. g. IrO2, Pt) with comparable electrochemical performance to the standard noble metal/metal oxide for proton exchange membrane (PEM) based water electrolysis would signify a major breakthrough in hydrogen generation via water electrolysis. Development of such systems would lead to two primary outcomes: first, a reduction in the overall capital costs of PEM based water electrolyzers, and second, attainment of the targeted hydrogen production costs (<$3.00/gge delivered by 2015) comparable to conventional liquid fuels. In line with these goals, by exploiting a two-pronged theoretical first principles and experimental approach herein, we demonstrate for the very first time a solid solution of SnO2:10 wt% F containing only 20 at.% IrO2 [e. g. (Sn0.80Ir0.20)O-2:10F] displaying remarkably similar electrochemical activity and comparable or even much improved electrochemical durability compared to pure IrO2, the accepted gold standard in oxygen evolution electro-catalysts for PEM based water electrolysis. We present the results of these studies. C1 [Datta, Moni Kanchan; Velikokhatnyi, Oleg I.; Kumta, Prashant N.] Univ Pittsburgh, Swanson Sch Engn, Dept Bioengn, Pittsburgh, PA 15261 USA. [Datta, Moni Kanchan; Velikokhatnyi, Oleg I.; Kumta, Prashant N.] Univ Pittsburgh, Ctr Complex Engn Multifunct Mat, Pittsburgh, PA 15261 USA. [Kadakia, Karan; Jampani, Prashanth H.; Kumta, Prashant N.] Univ Pittsburgh, Swanson Sch Engn, Pittsburgh, PA 15261 USA. [Chung, Sung Jae; Kumta, Prashant N.] Univ Pittsburgh, Pittsburgh, PA 15261 USA. [Poston, James A.; Manivannan, Ayyakkannu] US DOE, Natl Energy Technol Lab, Morgantown, WV 26507 USA. [Kumta, Prashant N.] Univ Pittsburgh, Sch Dent Med, Dept Oral Biol, Pittsburgh, PA 15217 USA. RP Datta, MK (reprint author), Univ Pittsburgh, Swanson Sch Engn, Dept Bioengn, Pittsburgh, PA 15261 USA. EM pkumta@pitt.edu RI Jampani Hanumantha, Prashanth/A-9840-2013 OI Jampani Hanumantha, Prashanth/0000-0001-7159-1993 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-SC0001531]; Edward R. Weidlein Chair Professorship funds FX Research supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under award DE-SC0001531. The authors also acknowledge Pittsburgh Supercomputing Center for allocation of computational resources. P.N.K. acknowledges the Edward R. Weidlein Chair Professorship funds and the Center for Complex Engineered Multifunctional Materials (CCEMM) for procuring the electrochemical equipment and facilities used in this research work. NR 42 TC 29 Z9 29 U1 3 U2 65 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2050-7488 J9 J MATER CHEM A JI J. Mater. Chem. A PY 2013 VL 1 IS 12 BP 4026 EP 4037 DI 10.1039/c3ta01458d PG 12 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Energy & Fuels; Materials Science GA 095TB UT WOS:000315356500028 ER PT J AU Ganusov, VV Neher, RA Perelson, AS AF Ganusov, Vitaly V. Neher, Richard A. Perelson, Alan S. TI Mathematical modeling of escape of HIV from cytotoxic T lymphocyte responses SO JOURNAL OF STATISTICAL MECHANICS-THEORY AND EXPERIMENT LA English DT Article DE dynamics (theory); models for evolution (theory); computational biology ID HUMAN-IMMUNODEFICIENCY-VIRUS; MHC CLASS-I; ANTIGEN PRESENTATION; SEXUAL POPULATIONS; RELATIVE FITNESS; RHESUS MACAQUES; VACCINE DESIGN; CTL ESCAPE; INFECTION; SELECTION AB Human immunodeficiency virus (HIV-1 or simply HIV) induces a persistent infection, which in the absence of treatment leads to AIDS and death in almost all infected individuals. HIV infection elicits a vigorous immune response starting about 2-3 weeks postinfection that can lower the amount of virus in the body, but which cannot eradicate the virus. How HIV establishes a chronic infection in the face of a strong immune response remains poorly understood. It has been shown that HIV is able to rapidly change its proteins via mutation to evade recognition by virus-specific cytotoxic T lymphocytes (CTLs). Typically, an HIV-infected patient will generate 4-12 CTL responses specific for parts of viral proteins called epitopes. Such CTL responses lead to strong selective pressure to change the viral sequences encoding these epitopes so as to avoid CTL recognition. Indeed, the viral population 'escapes' from about half of the CTL responses by mutation in the first year. Here we review experimental data on HIV evolution in response to CTL pressure, mathematical models developed to explain this evolution, and highlight problems associated with the data and previous modeling efforts. We show that estimates of the strength of the epitope-specific CTL response depend on the method used to fit models to experimental data and on the assumptions made regarding how mutants are generated during infection. We illustrate that allowing CTL responses to decay over time may improve the model fit to experimental data and provides higher estimates of the killing efficacy of HIV-specific CTLs. We also propose a novel method for simultaneously estimating the killing efficacy of multiple CTL populations specific for different epitopes of HIV using stochastic simulations. Lastly, we show that current estimates of the efficacy at which HIV-specific CTLs clear virus-infected cells can be improved by more frequent sampling of viral sequences and by combining data on sequence evolution with experimentally measured CTL dynamics. C1 [Ganusov, Vitaly V.] Univ Tennessee, Dept Microbiol, Knoxville, TN 37996 USA. [Neher, Richard A.] Max Planck Inst Dev Biol, D-72070 Tubingen, Germany. [Perelson, Alan S.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Ganusov, VV (reprint author), Univ Tennessee, Dept Microbiol, Knoxville, TN 37996 USA. EM richard.neher@tuebingen.mpg.de; asp@lanl.gov OI Ganusov, Vitaly/0000-0001-6572-1691; Neher, Richard/0000-0003-2525-1407 FU NSF [PHY05-51164]; US Department of Energy [DE-AC52-06NA25396]; NIH grant [R37-AI028433]; National Center for Research Resources; Office of Research Infrastructure Programs (ORIP) [8R01-OD011095-21]; ERC [260686] FX This work began with discussions between ASP and RAN at a Kavli Institute of Theoretical Physics workshop supported by NSF grant PHY05-51164. This work was performed under the auspices of the US Department of Energy under contract DE-AC52-06NA25396, and supported by NIH grant R37-AI028433 and the National Center for Research Resources and the Office of Research Infrastructure Programs (ORIP) through grant 8R01-OD011095-21 (ASP). RAN is supported by ERC Starting Grant no. 260686(HIVEVO). NR 53 TC 12 Z9 12 U1 2 U2 19 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1742-5468 J9 J STAT MECH-THEORY E JI J. Stat. Mech.-Theory Exp. PD JAN PY 2013 SI SI AR P01010 DI 10.1088/1742-5468/2013/01/P01010 PG 22 WC Mechanics; Physics, Mathematical SC Mechanics; Physics GA 096NF UT WOS:000315410500011 PM 24660019 ER PT J AU Song, MK Cairns, EJ Zhang, YG AF Song, Min-Kyu Cairns, Elton J. Zhang, Yuegang TI Lithium/sulfur batteries with high specific energy: old challenges and new opportunities SO NANOSCALE LA English DT Article ID COMPOSITE CATHODE MATERIALS; SULFUR BATTERIES; ELECTROCHEMICAL PROPERTIES; CARBON NANOTUBES; HIGH-CAPACITY; RECHARGEABLE BATTERIES; POLYMER ELECTROLYTES; ENCAPSULATED SULFUR; LIQUID ELECTROLYTE; CELL ELECTROLYTE AB In this review, we begin with a brief discussion of the operating principles and scientific/technical challenges faced by the development of lithium/sulfur cells. We then introduce some recent progress in exploring cathodes, anodes, and electrolytes for lithium/sulfur cells. In particular, several effective strategies used to enhance energy/power density, obtain good efficiencies, and prolong cycle life will be highlighted. We also discuss recent advancements in techniques for investigating electrode reactions in real time and monitoring structural/morphological changes of electrode materials under cell operating conditions to gain a better understanding of the mechanistic details of electrode processes. Finally, the opportunities and perspective for future research directions will be discussed. C1 [Song, Min-Kyu; Zhang, Yuegang] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Song, Min-Kyu; Cairns, Elton J.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Cairns, Elton J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Zhang, Yuegang] Chinese Acad Sci, Suzhou Inst Nanotech & Nanobion, Suzhou 215123, Peoples R China. RP Zhang, YG (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. EM yzhang5@lbl.gov RI Zhang, Y/E-6600-2011; Cairns, Elton/E-8873-2012 OI Zhang, Y/0000-0003-0344-8399; Cairns, Elton/0000-0002-1179-7591 NR 101 TC 195 Z9 199 U1 22 U2 346 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2040-3364 EI 2040-3372 J9 NANOSCALE JI Nanoscale PY 2013 VL 5 IS 6 BP 2186 EP 2204 DI 10.1039/c2nr33044j PG 19 WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 097ZM UT WOS:000315512000001 PM 23397572 ER PT J AU Li, GH Sundararajan, A Mouti, A Chang, YJ Lupini, AR Pennycook, SJ Strachan, DR Guiton, BS AF Li, Guohua Sundararajan, Abhishek Mouti, Anas Chang, Yao-Jen Lupini, Andrew R. Pennycook, Stephen J. Strachan, Douglas R. Guiton, Beth S. TI Synthesis and characterization of p-n homojunction-containing zinc oxide nanowires SO NANOSCALE LA English DT Article ID ABRUPT AXIAL HETEROJUNCTIONS; SOLAR-CELLS; SEMICONDUCTOR NANOWIRES; SILICON NANOWIRES; GROWTH; ARRAYS; JUNCTIONS; DIODES AB We illustrate a simple method to synthesize highly ordered ZnO axial p-n homojunction-containing nanowires using a low temperature method, and on a variety of substrates. X-ray diffraction, scanning transmission electron microscopy, scanning electron microscopy, and Raman spectroscopy are used to reveal high quality single-crystalline wires with a [001] growth direction. The study of electrical transport through a single nanowire based device and cathodoluminescence via scanning transmission electron microscopy demonstrates that an axial p-n junction exists within each ZnO nanowire. This represents the first low temperature synthesis of axial p-n homojunction-containing ZnO nanowires with uniform and controllable diameters. C1 [Li, Guohua; Mouti, Anas; Chang, Yao-Jen; Guiton, Beth S.] Univ Kentucky, Dept Chem, Lexington, KY 40506 USA. [Sundararajan, Abhishek; Strachan, Douglas R.] Univ Kentucky, Dept Phys & Astron, Lexington, KY 40506 USA. [Mouti, Anas; Lupini, Andrew R.; Pennycook, Stephen J.; Guiton, Beth S.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Pennycook, Stephen J.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. RP Guiton, BS (reprint author), Univ Kentucky, Dept Chem, Lexington, KY 40506 USA. EM beth.guiton@uky.edu RI Chang, Yao-Jen/E-6766-2017 FU Oak Ridge National Laboratory's Laboratory Directed Research and Development Fund; Office of Basic Energy Sciences, Materials Sciences and Engineering Division, U.S. Department of Energy; Kentucky NSF EPSCoR program through the Center of Advanced Materials FX Many thanks to Prof. P Stadelmann, Prof. C. Hebert and the CIME laboratory (Ecole Polytechnique Federale de Lausanne) for allowing us the use of their JEOL 2200FS STEM with CL detector. This research was supported by Oak Ridge National Laboratory's Laboratory Directed Research and Development Fund (AM, BSG), the Office of Basic Energy Sciences, Materials Sciences and Engineering Division, U.S. Department of Energy (SJP, ARL), and partially supported by the Kentucky NSF EPSCoR program through the Center of Advanced Materials (GL, DRS, BSG). NR 32 TC 13 Z9 13 U1 1 U2 86 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2040-3364 J9 NANOSCALE JI Nanoscale PY 2013 VL 5 IS 6 BP 2259 EP 2263 DI 10.1039/c3nr31639d PG 5 WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 097ZM UT WOS:000315512000008 PM 23403977 ER PT B AU Wiest, A Baker, SE McCluskey, K AF Wiest, Aric Baker, Scott E. McCluskey, Kevin BE Kasbekar, DP McCluskey, K TI Neurospora Gene and Genome Analysis: Past Through Future SO NEUROSPORA: GENOMICS AND MOLECULAR BIOLOGY LA English DT Article; Book Chapter ID 5S RIBOSOMAL-RNA; ELECTROPHORETIC KARYOTYPE; NUCLEOTIDE-SEQUENCE; CRASSA; CHROMOSOME; DNA; ORGANISM; MAP; IDENTIFICATION; INACTIVATION AB As modern biological research has developed, so has the analysis of Neurospora biology. From beginnings as a simple genetic system to the present where high throughput analysis enables questions in every area of biological inquiry, research on Neurospora continues to set a high standard for all filamentous fungal experimental systems. Analysis of materials developed over fifty years at the Fungal Genetics Stock Center (FGSC) using a variety of techniques including genetic mapping, cosmid walking, and gene and whole genome sequencing reveals both new information and reinforces discoveries made over many years. Neurospora is and will continue to be the premier organism for studies of the biology of filamentous fungi. C1 [Wiest, Aric; McCluskey, Kevin] Univ Missouri, Sch Biol Sci, Kansas City, MO 64110 USA. [Baker, Scott E.] Pacific NW Natl Lab, Chem & Biol Proc Dev Grp, Richland, WA 99352 USA. RP Wiest, A (reprint author), Univ Missouri, Sch Biol Sci, Kansas City, MO 64110 USA. EM wiesta@umkc.edu; scott.baker@pnnl.gov; mccluskeyk@umkc.edu NR 82 TC 0 Z9 0 U1 0 U2 1 PU CAISTER ACADEMIC PRESS PI WYMONDHAM PA 32 HEWITTS LANE, WYMONDHAM NR 18 0JA, ENGLAND BN 978-1-908230-12-6 PY 2013 BP 273 EP 289 PG 17 WC Biochemistry & Molecular Biology; Mycology SC Biochemistry & Molecular Biology; Mycology GA BDH84 UT WOS:000313301500015 ER PT J AU Kim, J Tsouris, C Oyola, Y Mayes, R Hexel, C Janke, C Dai, S AF Kim, Jungseung Tsouris, Costas Oyola, Yatsandra Mayes, Richard Hexel, Cole Janke, Christopher Dai, Sheng TI Adsorption tests SO NUCLEAR ENGINEERING INTERNATIONAL LA English DT Article C1 [Kim, Jungseung; Tsouris, Costas; Oyola, Yatsandra; Mayes, Richard; Hexel, Cole; Janke, Christopher; Dai, Sheng] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Kim, J (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RI Tsouris, Costas/C-2544-2016; Dai, Sheng/K-8411-2015; Hexel, Cole/N-3245-2016; Janke, Christopher/E-1598-2017 OI Tsouris, Costas/0000-0002-0522-1027; Dai, Sheng/0000-0002-8046-3931; Hexel, Cole/0000-0001-8101-2422; Janke, Christopher/0000-0002-6076-7188 FU US Department of Energy, Office of Nuclear Energy [DE-AC05-00OR22725]; Oak Ridge National Laboratory FX This work was sponsored by the US Department of Energy, Office of Nuclear Energy, under contract DE-AC05-00OR22725 with Oak Ridge National Laboratory, managed by UT-Battelle, LLC. References have been omitted for space but are available on www.neimagazine.com/seawateru NR 0 TC 12 Z9 12 U1 0 U2 6 PU WILMINGTON PUBL PI SIDCUP PA WILMINGTON HOUSE, MAIDSTONE RD, FOOTS CRAY, SIDCUP DA14 SHZ, KENT, ENGLAND SN 0029-5507 J9 NUCL ENG INT JI Nucl. Eng. Int. PD JAN PY 2013 VL 58 IS 702 BP 34 EP 35 PG 2 WC Nuclear Science & Technology SC Nuclear Science & Technology GA 097JV UT WOS:000315470900009 ER PT J AU Sosonkina, M Watson, LT Radcliffe, NR Haftka, RT Trosset, MW AF Sosonkina, Masha Watson, Layne T. Radcliffe, Nicholas R. Haftka, Rafael T. Trosset, Michael W. TI Adjusting process count on demand for petascale global optimization SO PARALLEL COMPUTING LA English DT Article DE Petascale; Message passing interface (MPI); Dynamic process count; Global optimization ID ADAPTIVE PARALLELISM; NOWS AB There are many challenges that need to be met before efficient and reliable computation at the petascale is possible. Many scientific and engineering codes running at the petascale are likely to be memory intensive, which makes thrashing a serious problem for many petascale applications. One way to overcome this challenge is to use a dynamic number of processes, so that the total amount of memory available for the computation can be increased on demand. This paper describes modifications made to the massively parallel global optimization code pVTdirect in order to allow for a dynamic number of processes. In particular, the modified version of the code monitors memory use and spawns new processes if the amount of available memory is determined to be insufficient. The primary design challenges are discussed, and performance results are presented and analyzed. (C) 2012 Elsevier B.V. All rights reserved. C1 [Sosonkina, Masha] Old Dominion Univ, Dept Modeling Simulat & Visualizat Engn, Norfolk, VA USA. [Sosonkina, Masha] Iowa State Univ, US DOE, Ames Lab, Ames, IA USA. [Watson, Layne T.; Radcliffe, Nicholas R.] Virginia Polytech Inst & State Univ, Dept Comp Sci, Blacksburg, VA 24061 USA. [Watson, Layne T.] Virginia Polytech Inst & State Univ, Dept Math, Blacksburg, VA 24061 USA. [Haftka, Rafael T.] Univ Florida, Dept Mech & Aerosp Engn, Gainesville, FL USA. [Trosset, Michael W.] Indiana Univ, Dept Stat, Bloomington, IN USA. RP Sosonkina, M (reprint author), Iowa State Univ, Old Dominion Univ, US DOE, Ames Lab, Ames, IA 50011 USA. EM msosonki@odu.edu; ltw@cs.vt.edu; nradclif@vt.edu; haftka@ufl.edu; mtrosset@indiana.edu FU AFOSR [FA9550-09-1-0153]; AFRL [FA8650-09-2-3938]; Ames Laboratory (Iowa State University) [DE-AC02-07CH11358]; U.S. Department of Energy, by Office of Science, Division of Mathematical, Information, and Computational Sciences of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported in part by AFOSR Grant FA9550-09-1-0153 and AFRL Grant FA8650-09-2-3938, in part by Ames Laboratory (Iowa State University) under the contract DE-AC02-07CH11358 with the U.S. Department of Energy, by the Director, Office of Science, Division of Mathematical, Information, and Computational Sciences of the U.S. Department of Energy under contract number DE-AC02-05CH11231. NR 22 TC 0 Z9 0 U1 1 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-8191 J9 PARALLEL COMPUT JI Parallel Comput. PD JAN PY 2013 VL 39 IS 1 BP 21 EP 35 DI 10.1016/j.parco.2012.11.001 PG 15 WC Computer Science, Theory & Methods SC Computer Science GA 098NZ UT WOS:000315557300002 ER PT J AU Mebane, DS Bhat, KS Kress, JD Fauth, DJ Gray, ML Lee, A Miller, DC AF Mebane, David S. Bhat, K. Sham Kress, Joel D. Fauth, Daniel J. Gray, McMahan L. Lee, Andrew Miller, David C. TI Bayesian calibration of thermodynamic models for the uptake of CO2 in supported amine sorbents using ab initio priors SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID CARBON-DIOXIDE CAPTURE; EXPANDED MESOPOROUS SILICA; CHAIN MONTE-CARLO; AQUEOUS-SOLUTIONS; MOLECULAR-SIEVE; IONIC LIQUIDS; HIGH-CAPACITY; ABSORPTION; ADSORPTION; SORPTION AB A statistical methodology was applied to the simultaneous calibration and validation of thermodynamic models for the uptake of CO2 in mesoporous silica-supported amines. The methodology is Bayesian, and follows the procedure introduced by Kennedy and O'Hagan. One key aspect of the application presented is the use of quantum chemical calculations to define prior probability distributions for physical model parameters. Inclusion of this prior information proved to be crucial to the identifiability of model parameters against experimental thermogravimetric data. Through the statistical analysis, a quantitative assessment of the accuracy of various quantum chemical methods is produced. Another important aspect of the current approach is the conditioning of the model form discrepancy - a critical component of the Kennedy and O'Hagan methodology - to the experimental data in such a mannner that it becomes an implicit function of the model parameters and thereby connected with the posterior distribution. It is shown that the inclusion of prior information in the analysis leads to a shifting of uncertainty from the posterior distribution for model parameters to this conditioned model form discrepancy. Prospects for more accurate model predictions and propagation of uncertainty in upscaling and extrapolation through a "model-plus-discrepancy" approach are discussed. The synthesis methods and thermogravimetric characterization of hybrid grafted/impregnated mesoporous silica-supported amine sorbents are presented, along with the details of the quantum chemical study, which shows that a carbamic acid-base acceptor complex is the most stable form of adsorbed CO2 in both alkanol- and ethyleneamines. C1 [Mebane, David S.; Fauth, Daniel J.; Gray, McMahan L.; Lee, Andrew; Miller, David C.] Natl Energy Technol Lab, Morgantown, WV USA. [Mebane, David S.; Fauth, Daniel J.; Gray, McMahan L.; Lee, Andrew; Miller, David C.] Natl Energy Technol Lab, Pittsburgh, PA USA. [Mebane, David S.] W Virginia Univ, Dept Mech & Aerosp Engn, Morgantown, WV 26506 USA. [Bhat, K. Sham; Kress, Joel D.] Los Alamos Natl Lab, Los Alamos, NM USA. RP Mebane, DS (reprint author), Natl Energy Technol Lab, Morgantown, WV USA. EM david.mebane@mail.wvu.edu RI Lee, Andrew/B-7019-2014 OI Lee, Andrew/0000-0002-0631-2537 FU ORISE postdoctoral fellowship; Department of Energy through the Carbon Capture Simulation Initiative; United States Government; National Nuclear Security Administration of the U.S. Department of Energy [DE-AC52-06NA25396] FX Partial support for David Mebane and Andrew Lee were provided through an ORISE postdoctoral fellowship.; Funding for this work was provided by the Department of Energy through the Carbon Capture Simulation Initiative.; This report was prepared as an account of work sponsored by an agency of the United States Government. Neither the United States Government nor any agency thereof, nor any of their employees, makes any warranty, express or implied, or assumes any legal liability or responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would not infringe privately owned rights. Reference herein to any specific commercial product, process, or service by trade name,trademark, manufacturer, or otherwise does not necessarily constitute or imply its endorsement, recommendation, or favoring by the United States Government or any agency thereof. The views and opinions of authors expressed herein do not necessarily state or reflect those of the United States Government or any agency thereof.; The Los Alamos National Laboratory is operated by Los Alamos National Security, LLC for the National Nuclear Security Administration of the U.S. Department of Energy under Contract No. DE-AC52-06NA25396. NR 66 TC 10 Z9 10 U1 0 U2 43 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PY 2013 VL 15 IS 12 BP 4355 EP 4366 DI 10.1039/c3cp42963f PG 12 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 096NM UT WOS:000315411200034 PM 23416704 ER PT J AU Hillesheim, PC Singh, JA Mahurin, SM Fulvio, PF Oyola, Y Zhu, X Jiang, DE Dai, S AF Hillesheim, Patrick C. Singh, Joseph A. Mahurin, Shannon M. Fulvio, Pasquale F. Oyola, Yatsandra Zhu, Xiang Jiang, De-en Dai, Sheng TI Effect of alkyl and aryl substitutions on 1,2,4-triazolium-based ionic liquids for carbon dioxide separation and capture SO RSC ADVANCES LA English DT Article ID THERMOPHYSICAL PROPERTIES; COSMO-RS; TRANSPORT-PROPERTIES; TRIAZOLIUM YLIDES; GAS SEPARATIONS; IMIDAZOLIUM; CO2; SOLUBILITY; SALTS; SOLVENTS AB A series of 1,2,4-triazolium-based ionic liquids have been synthesized and evaluated for their use in supported ionic liquid membrane based CO2 separations. The properties of these triazolium-based compounds have proven sensitive to isomeric substitutions, such as isopropyl and propyl groups, as well as ortho and para substitutions in the aryl derivative compounds. While physical properties such as viscosity did not vary significantly between structural isomers, the CO2 permeability, selectivity, and solubility exhibited significant changes allowing for development of task-specific triazolium-based ionic liquids for separation applications. OSMOtherm studies were also completed to gain a better understanding of the ionic liquids which demonstrated a strong correlation between experimental and computational values for the alkyl bearing ionic liquids. Hence, 1,2,4-triazolium-based liquids comprise a class of compounds offering unique opportunities to examine how structural changes affect the physicochemical properties which are necessary for the continuous development of ionic liquids with enhanced adsorption capacity and selectivity in separations. C1 [Hillesheim, Patrick C.; Singh, Joseph A.; Mahurin, Shannon M.; Fulvio, Pasquale F.; Oyola, Yatsandra; Jiang, De-en; Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Zhu, Xiang; Dai, Sheng] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. RP Hillesheim, PC (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. EM mahurinsm@ornl.gov; dais@ornl.gov RI Jiang, De-en/D-9529-2011; Fulvio, Pasquale/B-2968-2014; Zhu, Xiang/P-6867-2014; Dai, Sheng/K-8411-2015; OI Jiang, De-en/0000-0001-5167-0731; Fulvio, Pasquale/0000-0001-7580-727X; Zhu, Xiang/0000-0002-3973-4998; Dai, Sheng/0000-0002-8046-3931; Singh, Joseph/0000-0001-5249-2121 FU Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U. S. Department of Energy FX This work was fully sponsored by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U. S. Department of Energy. NR 57 TC 17 Z9 17 U1 1 U2 73 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2046-2069 J9 RSC ADV JI RSC Adv. PY 2013 VL 3 IS 12 BP 3981 EP 3989 DI 10.1039/c2ra22646d PG 9 WC Chemistry, Multidisciplinary SC Chemistry GA 095SS UT WOS:000315355600031 ER PT J AU Straub, TM Hutchison, JR Bartholomew, RA Valdez, CO Valentine, NB Dohnalkova, A Ozanich, RM Bruckner-Lea, CJ AF Straub, T. M. Hutchison, J. R. Bartholomew, R. A. Valdez, C. O. Valentine, N. B. Dohnalkova, A. Ozanich, R. M. Bruckner-Lea, C. J. TI Defining cell culture conditions to improve human norovirus infectivity assays SO WATER SCIENCE AND TECHNOLOGY LA English DT Article DE C2BBe1 cells; infectivity; noroviruses; qRT-PCR; three-dimensional cell culture ID BLOOD GROUP ANTIGENS; NORWALK VIRUS-RNA; MAMMALIAN-CELLS; DENDRITIC CELLS; PATHOGENESIS; BINDING; GASTROENTERITIS; REPLICATION; MACROPHAGES; REVEALS AB Significant difficulties remain for determining whether human noroviruses (hNoV) recovered from water, food, and environmental samples are infectious. Three-dimensional (3-D) tissue culture of human intestinal cells has shown promise in developing an infectivity assay, but reproducibility, even within a single laboratory, remains problematic. From the literature and our observations, we hypothesized that the common factors that lead to more reproducible hNoV infectivity in vitro requires that the cell line be (1) of human gastrointestinal origin, (2) expresses apical microvilli, and (3) be a positive secretor cell line. The C2BBe1 cell line, which is a brush-border producing clone of Caco-2, meets these three criteria. When challenged with Genogroup II viruses, we observed a 2 Log(10) increase in viral RNA titer. A passage experiment with GII viruses showed evidence of the ability to propagate hNoV by both quantitative reverse transcription polymerase chain reaction (qRT-PCR) and microscopy. In our hands, using 3-D C2BBe1 cells improves reproducibility of the infectivity assay for hNoV, but the assay can still be variable. Two sources of variability include the cells themselves (mixed phenotypes of small and large intestine) and initial titer measurements using qRT-PCR that measures all RNA vs. plaque assays that measure infectious virus. C1 [Straub, T. M.; Hutchison, J. R.; Bartholomew, R. A.; Valdez, C. O.; Valentine, N. B.; Dohnalkova, A.; Ozanich, R. M.; Bruckner-Lea, C. J.] Pacific NW Natl Lab, Richland, WA 99354 USA. RP Straub, TM (reprint author), Pacific NW Natl Lab, 902 Battelle Blvd,MS P7-50, Richland, WA 99354 USA. EM Timothy.Straub@pnnl.gov FU National Institute of Allergy and Infectious Diseases, National Institutes of Health, Department of Health and Human Services [NO1-AI-30055]; United States Environmental Protection Agency STAR Grant Program [R833831010]; United States Department of Energy Laboratory Directed Research and Development (LDRD) grant; Department of Energy's Office of Biological and Environmental Research located at Pacific Northwest National Laboratory; United States Department of Energy [DE-AC06-76RLO 1830] FX The authors wish to thank William Chrisler for his assistance with confocal microscopy (Figure 1(a)). This research was funded in part by the National Institute of Allergy and Infectious Diseases, National Institutes of Health, Department of Health and Human Services, under contract no. NO1-AI-30055 and the United States Environmental Protection Agency STAR Grant Program (Grant R833831010). Confocal and scanning electron microscopy was funded in part by the United States Department of Energy Laboratory Directed Research and Development (LDRD) grant for J. R. Hutchison as part of a human microbiome community preliminary study. A portion of this research was performed using EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research located at Pacific Northwest National Laboratory. PNNL is operated by Battelle Memorial Institute for the United States Department of Energy under contract DE-AC06-76RLO 1830. NR 25 TC 9 Z9 9 U1 2 U2 21 PU IWA PUBLISHING PI LONDON PA ALLIANCE HOUSE, 12 CAXTON ST, LONDON SW1H0QS, ENGLAND SN 0273-1223 J9 WATER SCI TECHNOL JI Water Sci. Technol. PY 2013 VL 67 IS 4 BP 863 EP 868 DI 10.2166/wst.2012.636 PG 6 WC Engineering, Environmental; Environmental Sciences; Water Resources SC Engineering; Environmental Sciences & Ecology; Water Resources GA 093MB UT WOS:000315194900022 PM 23306266 ER PT J AU Plasser, F Pasalic, H Gerzabek, MH Libisch, F Reiter, R Burgdorfer, J Muller, T Shepard, R Lischka, H AF Plasser, Felix Pasalic, Hasan Gerzabek, Martin H. Libisch, Florian Reiter, Rafael Burgdoerfer, Joachim Mueller, Thomas Shepard, Ron Lischka, Hans TI The Multiradical Character of One- and Two-Dimensional Graphene Nanoribbons SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE chemical stability; graphene; multiradical character; multireference methods; quantum chemistry ID CHARACTERIZING UNPAIRED ELECTRONS; PARTICLE DENSITY-MATRIX; COUPLED-CLUSTER; GROUND-STATE; ACENES; PHOTOGENERATION; HEPTACENE; SIZE C1 [Plasser, Felix; Pasalic, Hasan; Lischka, Hans] Univ Vienna, Inst Theoret Chem, A-1090 Vienna, Austria. [Gerzabek, Martin H.] Univ Nat Resources & Life Sci, Inst Soil Res, A-1190 Vienna, Austria. [Libisch, Florian; Reiter, Rafael; Burgdoerfer, Joachim] Vienna Univ Technol, Inst Theoret Phys, A-1040 Vienna, Austria. [Mueller, Thomas] Forschungszentrum Julich, Inst Adv Simulat, Julich Supercomp Ctr, D-52425 Julich, Germany. [Shepard, Ron] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Lischka, Hans] Texas Tech Univ, Dept Chem & Biochem, Lubbock, TX 79409 USA. RP Lischka, H (reprint author), Univ Vienna, Inst Theoret Chem, Waehringerstr 17, A-1090 Vienna, Austria. EM hans.lischka@univie.ac.at RI Lischka, Hans/A-8802-2015; Plasser, Felix/C-1149-2013; OI Plasser, Felix/0000-0003-0751-148X; Libisch, Florian/0000-0001-5641-9458 FU Austrian Science Fund [SFB F41, P20893-N19]; Deutsche Forschungsgemeinschaft [SPP 1315, GE1676/1-1]; Robert A. Welch Foundation [D-0005]; Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences, U.S. Department of Energy [DE-AC02-06CH11357]; [70151] FX This work was supported by the Austrian Science Fund (SFB F41, ViCoM, and Project P20893-N19), the Deutsche Forschungsgemeinschaft (SPP 1315, Project GE1676/1-1), the Robert A. Welch Foundation (grant no. D-0005), and the Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences, U.S. Department of Energy (contract number DE-AC02-06CH11357 to H.L. and R.S.). We are grateful to T.J. Mach and T.D. Crawford for implementation of the D2 diagnostic into PSI4 and for performing the respective calculations, as well as to the Vienna Scientific Cluster (VSC), Project 70151 for computer time. NR 39 TC 84 Z9 84 U1 6 U2 95 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PY 2013 VL 52 IS 9 BP 2581 EP 2584 DI 10.1002/anie.201207671 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA 093RR UT WOS:000315209900039 PM 23355507 ER PT J AU Palancar, GG Lefer, BL Hall, SR Shaw, WJ Corr, CA Herndon, SC Slusser, JR Madronich, S AF Palancar, G. G. Lefer, B. L. Hall, S. R. Shaw, W. J. Corr, C. A. Herndon, S. C. Slusser, J. R. Madronich, S. TI Effect of aerosols and NO2 concentration on ultraviolet actinic flux near Mexico City during MILAGRO: measurements and model calculations SO ATMOSPHERIC CHEMISTRY AND PHYSICS LA English DT Article ID PHOTOCHEMICAL SMOG; PHOTOLYSIS RATES; OZONE PRODUCTION; CLOUDY ATMOSPHERES; RADIATIVE-TRANSFER; METROPOLITAN-AREA; NITROGEN-OXIDES; 2006 CAMPAIGN; URBAN; SENSITIVITY AB Urban air pollution absorbs and scatters solar ultraviolet (UV) radiation, and thus has a potentially large effect on tropospheric photochemical rates. We present the first detailed comparison between actinic fluxes (AF) in the wavelength range 330-420 nm measured in highly polluted conditions and simulated with the Tropospheric Ultraviolet-Visible (TUV) model. Measurements were made during the MILAGRO campaign near Mexico City in March 2006, at a ground-based station near Mexico City (the T1 supersite) and from the NSF/NCAR C-130 aircraft. At the surface, measured AF values are typically smaller than the model by up to 25% in the morning, 10% at noon, and 40% in the afternoon, for pollution-free and cloud-free conditions. When measurements of PBL height, NO2 concentration and aerosols optical properties are included in the model, the agreement improves to within +/- 10% in the morning and afternoon, and +/- 3% at noon. Based on daily averages, aerosols account for 68% and NO2 for 25% of AF reductions observed at the surface. Several overpasses from the C-130 aircraft provided the opportunity to examine the AF perturbations aloft, and also show better agreement with the model when aerosol and NO2 effects are included above and below the flight altitude. TUV model simulations show that the vertical structure of the actinic flux is sensitive to the choice of the aerosol single scattering albedo (SSA) at UV wavelengths. Typically, aerosols enhance AF above the PBL and reduce AF near the surface. However, for highly scattering aerosols (SSA > 0.95), enhancements can penetrate well into the PBL, while for strongly absorbing aerosols (SSA < 0.6) reductions in AF are computed in the free troposphere as well as in the PBL. Additional measurements of the SSA at these wavelengths are needed to better constrain the effect of aerosols on the vertical structure of the AF. C1 [Palancar, G. G.; Hall, S. R.; Madronich, S.] Natl Ctr Atmospher Res, Div Atmospher Chem, Boulder, CO 80307 USA. [Palancar, G. G.] Univ Nacl Cordoba, Fac Ciencias Quim, Dept Quim Fis, Ctr Laser Ciencias Mol,INFIQC,CONICET, RA-5000 Cordoba, Argentina. [Lefer, B. L.] Univ Houston, Dept Earth & Atmospher Sci, Houston, TX USA. [Shaw, W. J.] US DOE, Pacific NW Natl Lab, Richland, WA USA. [Corr, C. A.] Univ New Hampshire, Earth Syst Res Ctr, Durham, NH 03824 USA. [Herndon, S. C.] Aerodyne Res Inc, Billerica, MA 01821 USA. [Slusser, J. R.] Colorado State Univ, UV B Monitoring & Res Program, USDA, Ft Collins, CO 80523 USA. RP Madronich, S (reprint author), Natl Ctr Atmospher Res, Div Atmospher Chem, Boulder, CO 80307 USA. EM sasha@ucar.edu RI Madronich, Sasha/D-3284-2015 OI Madronich, Sasha/0000-0003-0983-1313 FU CONICET; National Science Foundation; USDA/CSREES [2006-34263-16326]; NSF [ATM-0511911] FX G. G. Palancar would like to thank CONICET for an external fellowship. The National Center for Atmospheric Research is sponsored by the National Science Foundation. We thank AERONET principal investigator Brent Holben and his staff for their efforts in establishing and maintaining the T1_MAX_MEX site. The authors would like to thank R. C. Cohen (University of California, Berkeley) for providing the NO2 data at surface (LIF) and also to D. J. Knapp, D. D. Montzka, and A. J. Weinheimer (NCAR) for providing the NO2 measurements taken aboard the C-130 aircraft. Irradiance measurements were provided by the USDA UV-B Monitoring and Research Program supported by USDA/CSREES grant 2006-34263-16326, with additional support from NSF under grant number ATM-0511911. NR 59 TC 5 Z9 5 U1 2 U2 32 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1680-7316 J9 ATMOS CHEM PHYS JI Atmos. Chem. Phys. PY 2013 VL 13 IS 2 BP 1011 EP 1022 DI 10.5194/acp-13-1011-2013 PG 12 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 079LP UT WOS:000314172200031 ER PT J AU Kuai, L Worden, J Kulawik, S Bowman, K Lee, M Biraud, SC Abshire, JB Wofsy, SC Natraj, V Frankenberg, C Wunch, D Connor, B Miller, C Roehl, C Shia, RL Yung, Y AF Kuai, L. Worden, J. Kulawik, S. Bowman, K. Lee, M. Biraud, S. C. Abshire, J. B. Wofsy, S. C. Natraj, V. Frankenberg, C. Wunch, D. Connor, B. Miller, C. Roehl, C. Shia, R. -L. Yung, Y. TI Profiling tropospheric CO2 using Aura TES and TCCON instruments SO ATMOSPHERIC MEASUREMENT TECHNIQUES LA English DT Article ID COLUMN OBSERVING NETWORK; ATMOSPHERIC CO2; EMISSION SPECTROMETER; CARBON-DIOXIDE; RETRIEVAL ALGORITHM; GREENHOUSE GASES; GEOS-CHEM; CALIBRATION; SPACE; COVARIANCE AB Monitoring the global distribution and long-term variations of CO2 sources and sinks is required for characterizing the global carbon budget. Total column measurements are useful for estimating regional-scale fluxes; however, model transport remains a significant error source, particularly for quantifying local sources and sinks. To improve the capability of estimating regional fluxes, we estimate lower tropospheric CO2 concentrations from ground-based near-infrared (NIR) measurements with space-based thermal infrared (TIR) measurements. The NIR measurements are obtained from the Total Carbon Column Observing Network (TCCON) of solar measurements, which provide an estimate of the total CO2 column amount. Estimates of tropospheric CO2 that are co-located with TCCON are obtained by assimilating Tropospheric Emission Spectrometer (TES) free tropospheric CO2 estimates into the GEOS-Chem model. We find that quantifying lower tropospheric CO2 by subtracting free tropospheric CO2 estimates from total column estimates is a linear problem, because the calculated random uncertainties in total column and lower tropospheric estimates are consistent with actual uncertainties as compared to aircraft data. For the total column estimates, the random uncertainty is about 0.55 ppm with a bias of -5.66 ppm, consistent with previously published results. After accounting for the total column bias, the bias in the lower tropospheric CO2 estimates is 0.26 ppm with a precision (one standard deviation) of 1.02 ppm. This precision is sufficient for capturing the winter to summer variability of approximately 12 ppm in the lower troposphere; double the variability of the total column. This work shows that a combination of NIR and TIR measurements can profile CO2 with the precision and accuracy needed to quantify lower tropospheric CO2 variability. C1 [Kuai, L.; Worden, J.; Kulawik, S.; Bowman, K.; Lee, M.; Natraj, V.; Frankenberg, C.; Miller, C.] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Biraud, S. C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Abshire, J. B.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Wofsy, S. C.] Harvard Univ, Cambridge, MA 02138 USA. [Wunch, D.; Roehl, C.; Shia, R. -L.; Yung, Y.] CALTECH, Pasadena, CA 91125 USA. [Connor, B.] BC Consulting Ltd, Alexandra 9320, New Zealand. RP Kuai, L (reprint author), CALTECH, Jet Prop Lab, 4800 Oak Grove Dr,Mail Stop 233-200, Pasadena, CA 91109 USA. EM lkuai@jpl.nasa.gov RI Abshire, James/I-2800-2013; Biraud, Sebastien/M-5267-2013; Chem, GEOS/C-5595-2014; Frankenberg, Christian/A-2944-2013 OI Biraud, Sebastien/0000-0001-7697-933X; Frankenberg, Christian/0000-0002-0546-5857 FU NASA's Terrestrial Ecology Program [NNX11AG01G]; Orbiting Carbon Observatory Program; Atmospheric CO2 Observations from Space (ACOS) Program; DOE/ARM Program; Office of Biological and Environmental Research of the US Department of Energy, Atmospheric Radiation Measurement Program [DE-AC02-05CH11231]; [09-ACOS09-0010] FX Part of this research was carried out at the Jet Propulsion Laboratory, California Institute of Technology, under a contract with the National Aeronautics and Space Administration. The GEOS-Chem model results with assimilated TES data was funded by proposal No. 09-ACOS09-0010. US funding for TCCON comes from NASA's Terrestrial Ecology Program, grant number NNX11AG01G, the Orbiting Carbon Observatory Program, the Atmospheric CO2 Observations from Space (ACOS) Program and the DOE/ARM Program. SGP data was supported by the Office of Biological and Environmental Research of the US Department of Energy under contract No. DE-AC02-05CH11231 as part of the Atmospheric Radiation Measurement Program. The authors wish to thank G. Toon and P. Wennberg for making available their GFIT code and TCCON data. NR 63 TC 9 Z9 11 U1 1 U2 25 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1867-1381 J9 ATMOS MEAS TECH JI Atmos. Meas. Tech. PY 2013 VL 6 IS 1 BP 63 EP 79 DI 10.5194/amt-6-63-2013 PG 17 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 093FF UT WOS:000315176400006 ER PT J AU Appel, AA Chou, CY Larson, JC Zhong, Z Schoen, FJ Johnston, CM Brey, EM Anastasio, MA AF Appel, A. A. Chou, C-Y Larson, J. C. Zhong, Z. Schoen, F. J. Johnston, C. M. Brey, E. M. Anastasio, M. A. TI An initial evaluation of analyser-based phase-contrast X-ray imaging of carotid plaque microstructure SO BRITISH JOURNAL OF RADIOLOGY LA English DT Article ID HUMAN ATHEROSCLEROTIC PLAQUES; MAGNETIC-RESONANCE; INTRAPLAQUE HEMORRHAGE; ARTICULAR-CARTILAGE; IMAGES; IMPLEMENTATION; RADIOGRAPHY; HISTOLOGY; ARTERY; MRI AB Carotid artery plaque instability can result in rupture and lead to ischaemic stroke. Stability of plaques appears to be a function of composition. Current non-invasive imaging techniques are limited in their ability to classify distinct histological regions within plaques. Phase-contrast (PC) X-ray imaging methods are an emerging class of techniques that have shown promise for identifying soft-tissue features without use of exogenous contrast agents. This is the first study to apply analyser-based X-ray PC imaging in CT mode to provide three-dimensional (3D) images of excised atherosclerotic plaques. The results provide proof of principle for this technique as a promising method for analysis of carotid plaque microstructure. Multiple image radiography CT (MIR-CT), a tomographic implementation of X-ray PC imaging that employs crystal optics, was employed to image excised carotid plaques. MIR-CT imaging yields three complementary images of the plaque's 3D X-ray absorption, refraction and scatter properties. These images were compared with histological sections of the tissue. X-ray PC images were able to identify the interface between the plaque and the medial wall. In addition, lipid-rich and highly vascularized regions were visible in the images as well as features depicting inflammation. This preliminary research shows MIR-CT imaging can reveal details about plaque structure not provided by traditional absorption-based X-ray imaging and appears to identify specific histological regions within plaques. This is the first study to apply analyser-based X-ray PC imaging to human carotid artery plaques to identify distinct soft-tissue regions. C1 [Appel, A. A.; Larson, J. C.; Brey, E. M.] IIT, Dept Biomed Engn, Chicago, IL 60616 USA. [Appel, A. A.; Brey, E. M.] Hines VA Hosp, Dept Res, Hines, IL USA. [Chou, C-Y] Natl Taiwan Univ, Dept Bioind Mechatron Engn, Taipei 10764, Taiwan. [Zhong, Z.] Brookhaven Natl Lab, Natl Synchrotron Light Source, Upton, NY 11973 USA. [Schoen, F. J.] Brigham & Womens Hosp, Dept Pathol, Boston, MA 02115 USA. [Johnston, C. M.] Univ Texas MD Anderson Canc Ctr, Div Surg Core Histol Lab, Houston, TX 77030 USA. [Brey, E. M.] Washington Univ, Dept Biomed Engn, St Louis, MO USA. RP Brey, EM (reprint author), 3255 S Dearborn St,Wishnick Hall,Suite 314, Chicago, IL 60616 USA. EM brey@iit.edu OI CHOU, CHENG-YING/0000-0002-5737-6960 FU NIH [EB009715]; National Science Foundation [CBET 1135068]; Veterans Administration FX This research was supported by NIH grant EB009715, National Science Foundation grant CBET 1135068 and Veterans Administration. NR 29 TC 4 Z9 5 U1 1 U2 10 PU BRITISH INST RADIOLOGY PI LONDON PA 36 PORTLAND PLACE, LONDON W1N 4AT, ENGLAND SN 0007-1285 J9 BRIT J RADIOL JI Br. J. Radiol. PD JAN PY 2013 VL 86 IS 1021 AR UNSP 20120318 DI 10.1259/bjr.20120318 PG 6 WC Radiology, Nuclear Medicine & Medical Imaging SC Radiology, Nuclear Medicine & Medical Imaging GA 094MG UT WOS:000315266900022 PM 23239697 ER PT J AU Custelcean, R AF Custelcean, Radu TI Urea-functionalized crystalline capsules for recognition and separation of tetrahedral oxoanions SO CHEMICAL COMMUNICATIONS LA English DT Article ID METAL-ORGANIC FRAMEWORKS; HYDROGEN-BONDING GROUPS; ANION-BINDING; SELECTIVE CRYSTALLIZATION; CRYSTALLOGRAPHIC EVIDENCE; SULFATE RECOGNITION; TRIPODAL RECEPTOR; PHOSPHATE ANION; ENCAPSULATION; ION AB The persistent ability of tripodal TREN-based tris-urea receptors (TREN = tris(2-aminoethyl) amine) to self-assemble with a variety of oxoanions into dimeric capsules upon crystallization is reviewed. The capsule crystallization allows for charge-, shape-, and size-selective encapsulation of tetrahedral XO4n anions (n = 2,3), and provides an effective way to separate these anions from competitive aqueous environments. C1 Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. RP Custelcean, R (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. EM custelceanr@ornl.gov RI Custelcean, Radu/C-1037-2009 OI Custelcean, Radu/0000-0002-0727-7972 FU Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy FX This research was sponsored by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy. I would like to thank my coworkers and collaborators, particularly Bruce Moyer, Ben Hay, Peter Bonnesen, Priscilla Remy, Aurelien Bock, and Arbin Rajbanshi, who made significant contributions to the capsule crystallization project of our group over the last eight years. NR 88 TC 47 Z9 47 U1 3 U2 71 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1359-7345 J9 CHEM COMMUN JI Chem. Commun. PY 2013 VL 49 IS 22 BP 2173 EP 2182 DI 10.1039/c2cc38252k PG 10 WC Chemistry, Multidisciplinary SC Chemistry GA 093CH UT WOS:000315168800001 PM 23340607 ER PT J AU Mulfort, KL Mukherjee, A Kokhan, O Du, PW Tiede, DM AF Mulfort, Karen L. Mukherjee, Anusree Kokhan, Oleksandr Du, Pingwu Tiede, David M. TI Structure-function analyses of solar fuels catalysts using in situ X-ray scattering SO CHEMICAL SOCIETY REVIEWS LA English DT Review ID PHOTOCATALYTIC HYDROGEN-PRODUCTION; WATER-OXIDATION CATALYST; MOLECULAR-DYNAMICS; ARTIFICIAL PHOTOSYNTHESIS; COBALOXIME CATALYSTS; HOMOGENEOUS SYSTEM; COBALT CATALYST; H-2 PRODUCTION; COMPLEXES; EVOLUTION AB This tutorial review illustrates opportunities for the resolution of structure-function relationships to aid in the development of new materials for solar energy conversion using a combination of spectroscopy and catalysis measurements with X-ray scattering analyses to provide in situ structural characterization of solar fuels catalysts. As an example, the use of molecular cobaloxime catalysts in bimolecular and supramolecular photocatalysis schemes for proton reduction is briefly reviewed. These highlight the need to develop new modular, hierarchical, self-healing supramolecular architectures for solar fuels catalysis. Examples of the X-ray scattering structural analysis of amorphous materials in the context of photocatalytic function are discussed in detail. C1 [Mulfort, Karen L.; Mukherjee, Anusree; Kokhan, Oleksandr; Du, Pingwu; Tiede, David M.] Argonne Natl Lab, Div Chem Sci & Engn, Argonne, IL 60439 USA. RP Mulfort, KL (reprint author), Argonne Natl Lab, Div Chem Sci & Engn, 9700 S Cass Ave, Argonne, IL 60439 USA. EM mulfort@anl.gov; tiede@anl.gov RI Du, Pingwu/G-3329-2010; OI Du, Pingwu/0000-0002-2715-0979; Kokhan, Oleksandr/0000-0001-9867-8044 FU Division of Chemical Sciences, Biosciences, Office of Basic Energy Sciences of the U. S. Department of Energy [DE-AC02-06CH11357]; Argonne Northwestern Solar Research Center, an Energy Frontier Research Center; U.S. DOE, Office of Science, Office of Basic Energy Sciences [DE-SC0001059]; US DOE [DE-AC02-06CH11357] FX We gratefully acknowledge funding from the Division of Chemical Sciences, Biosciences, Office of Basic Energy Sciences of the U. S. Department of Energy through Grant DE-AC02-06CH11357 for support of the work on the supramolecular solar photocatalysts and the Co-OEC characterization. Work on the IrCp* complexes, collaboratively provided by J. Blakemore, G. Brudvig, R. Crabtree (Yale University), was supported as part of the Argonne Northwestern Solar Research Center, an Energy Frontier Research Center funded by the U.S. DOE, Office of Science, Office of Basic Energy Sciences under Award Number DE-SC0001059. This work benefited from the use of beamlines 12-ID-B and 11-ID-B of the Advanced Photon Source, a US DOE Office of Science User Facility, supported under US DOE Contract No. DE-AC02-06CH11357. NR 71 TC 21 Z9 21 U1 6 U2 109 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 0306-0012 EI 1460-4744 J9 CHEM SOC REV JI Chem. Soc. Rev. PY 2013 VL 42 IS 6 BP 2215 EP 2227 DI 10.1039/c2cs35247h PG 13 WC Chemistry, Multidisciplinary SC Chemistry GA 095SZ UT WOS:000315356300002 PM 23120752 ER PT J AU Thoi, VS Sun, YJ Long, JR Chang, CJ AF Thoi, V. Sara Sun, Yujie Long, Jeffrey R. Chang, Christopher J. TI Complexes of earth-abundant metals for catalytic electrochemical hydrogen generation under aqueous conditions SO CHEMICAL SOCIETY REVIEWS LA English DT Review ID IRON-ONLY HYDROGENASE; HYDROPHILIC PHOSPHATRIAZAADAMANTANE LIGAND; MOLYBDENUM-OXO CATALYST; H-2 PRODUCTION; ACTIVE-SITE; ELECTROCATALYTIC REDUCTION; MOLECULAR-HYDROGEN; COBALT CLATHROCHELATE; OXIDATIVE ADDITION; LOW OVERPOTENTIALS AB Growing global energy demands and climate change motivate the development of new renewable energy technologies. In this context, water splitting using sustainable energy sources has emerged as an attractive process for carbon-neutral fuel cycles. A key scientific challenge to achieving this overall goal is the invention of new catalysts for the reductive and oxidative conversions of water to hydrogen and oxygen, respectively. This review article will highlight progress in molecular electrochemical approaches for catalytic reduction of protons to hydrogen, focusing on complexes of earth-abundant metals that can function in pure aqueous or mixed aqueous-organic media. The use of water as a reaction medium has dual benefits of maintaining high substrate concentration as well as minimizing the environmental impact from organic additives and by-products. C1 [Thoi, V. Sara; Sun, Yujie; Long, Jeffrey R.; Chang, Christopher J.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Thoi, V. Sara; Sun, Yujie; Chang, Christopher J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Long, Jeffrey R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Chang, Christopher J.] Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA. RP Long, JR (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM jrlong@berkeley.edu; chrischang@berkeley.edu RI Sun, Yujie/A-9428-2012 FU DOE/LBNL [403801]; Joint Center for Artificial Photosynthesis, a DOE Energy Innovation Hub Office of Science of the U.S. Department of Energy [DE-SC0004993]; National Science Foundation for a Graduate Research Fellowship FX Our work in sustainable energy catalysis is supported by DOE/LBNL Grant 403801 (C.J.C.) and the Joint Center for Artificial Photosynthesis, a DOE Energy Innovation Hub, supported through the Office of Science of the U.S. Department of Energy under award DE-SC0004993 (J.R.L.). V. S. T. thanks the National Science Foundation for a Graduate Research Fellowship. C.J.C. is an Investigator with the Howard Hughes Medical Institute. NR 105 TC 220 Z9 220 U1 32 U2 346 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 0306-0012 EI 1460-4744 J9 CHEM SOC REV JI Chem. Soc. Rev. PY 2013 VL 42 IS 6 BP 2388 EP 2400 DI 10.1039/c2cs35272a PG 13 WC Chemistry, Multidisciplinary SC Chemistry GA 095SZ UT WOS:000315356300012 PM 23034627 ER PT J AU An, FP An, Q Bai, JZ Balantekin, AB Band, HR Beriguete, W Bishai, M Blyth, S Brown, RL Cao, GF Cao, J Carr, R Chan, WT Chang, JF Chang, Y Chasman, C Chen, HS Chen, HY Chen, SJ Chen, SM Chen, XC Chen, XH Chen, XS Chen, Y Chen, YX Cherwinka, JJ Chu, MC Cummings, JP Deng, ZY Ding, YY Diwan, MV Draeger, E Du, XF Dwyer, D Edwards, WR Ely, SR Fang, SD Fu, JY Fu, ZW Ge, LQ Gill, RL Gonchar, M Gong, GH Gong, H Gornushkin, YA Gu, WQ Guan, MY Guo, XH Hackenburg, RW Hahn, RL Hans, S Hao, HF He, M He, Q Heeger, KM Heng, YK Hinrichs, P Hor, YK Hsiung, YB Hu, BZ Hu, T Huang, HX Huang, HZ Huang, XT Huber, P Issakov, V Isvan, Z Jaffe, DE Jetter, S Ji, XL Ji, XP Jiang, HJ Jiao, JB Johnson, RA Kang, L Kettell, SH Kramer, M Kwan, KK Kwok, MW Kwok, T Lai, CY Lai, WC Lai, WH Lau, K Lebanowski, L Lee, J Lei, RT Leitner, R Leung, JKC Leung, KY Lewis, CA Li, F Li, GS Li, QJ Li, WD Li, XB Li, XN Li, XQ Li, Y Li, ZB Liang, H Lin, CJ Lin, GL Lin, SK Lin, YC Ling, JJ Link, JM Littenberg, L Littlejohn, BR Liu, DW Liu, JC Liu, JL Liu, YB Lu, C Lu, HQ Luk, A Luk, KB Ma, QM Ma, XB Ma, XY Ma, YQ McDonald, KT McFarlane, MC McKeown, RD Meng, Y Mohapatra, D Nakajima, Y Napolitano, J Naumov, D Nemchenok, I Ngai, HY Ngai, WK Nie, YB Ning, Z Ochoa-Ricoux, JP Olshevski, A Patton, S Pec, V Peng, JC Piilonen, LE Pinsky, L Pun, CSJ Qi, FZ Qi, M Qian, X Raper, N Ren, J Rosero, R Roskovec, B Ruan, XC Shao, BB Shih, K Steiner, H Sun, GX Sun, JL Tagg, N Tam, YH Tanaka, HK Tang, X Themann, H Torun, Y Trentalange, S Tsai, O Tsang, KV Tsang, RHM Tull, CE Tung, YC Viren, B Vorobel, V Wang, CH Wang, LS Wang, LY Wang, LZ Wang, M Wang, NY Wang, RG Wang, W Wang, X Wang, YF Wang, Z Wang, Z Wang, ZM Webber, DM Wei, HY Wei, YD Wen, LJ Whisnant, K White, CG Whitehead, L Williamson, Y Wise, T Wong, HLH Worcester, ET Wu, FF Wu, Q Xi, JB Xia, DM Xing, ZZ Xu, J Xu, J Xu, JL Xu, Y Xue, T Yang, CG Yang, L Ye, M Yeh, M Yeh, YS Young, BL Yu, ZY Zhan, L Zhang, C Zhang, FH Zhang, JW Zhang, QM Zhang, SH Zhang, YC Zhang, YH Zhang, YX Zhang, ZJ Zhang, ZP Zhang, ZY Zhao, J Zhao, QW Zhao, YB Zheng, L Zhong, WL Zhou, L Zhou, ZY Zhuang, HL Zou, JH AF An, F. P. An, Q. Bai, J. Z. Balantekin, A. B. Band, H. R. Beriguete, W. Bishai, M. Blyth, S. Brown, R. L. Cao, G. F. Cao, J. Carr, R. Chan, W. T. Chang, J. F. Chang, Y. Chasman, C. Chen, H. S. Chen, H. Y. Chen, S. J. Chen, S. M. Chen, X. C. Chen, X. H. Chen, X. S. Chen, Y. Chen, Y. X. Cherwinka, J. J. Chu, M. C. Cummings, J. P. Deng, Z. Y. Ding, Y. Y. Diwan, M. V. Draeger, E. Du, X. F. Dwyer, D. Edwards, W. R. Ely, S. R. Fang, S. D. Fu, J. Y. Fu, Z. W. Ge, L. Q. Gill, R. L. Gonchar, M. Gong, G. H. Gong, H. Gornushkin, Y. A. Gu, W. Q. Guan, M. Y. Guo, X. H. Hackenburg, R. W. Hahn, R. L. Hans, S. Hao, H. F. He, M. He, Q. Heeger, K. M. Heng, Y. K. Hinrichs, P. Hor, Y. K. Hsiung, Y. B. Hu, B. Z. Hu, T. Huang, H. X. Huang, H. Z. Huang, X. T. Huber, P. Issakov, V. Isvan, Z. Jaffe, D. E. Jetter, S. Ji, X. L. Ji, X. P. Jiang, H. J. Jiao, J. B. Johnson, R. A. Kang, L. Kettell, S. H. Kramer, M. Kwan, K. K. Kwok, M. W. Kwok, T. Lai, C. Y. Lai, W. C. Lai, W. H. Lau, K. Lebanowski, L. Lee, J. Lei, R. T. Leitner, R. Leung, J. K. C. Leung, K. Y. Lewis, C. A. Li, F. Li, G. S. Li, Q. J. Li, W. D. Li, X. B. Li, X. N. Li, X. Q. Li, Y. Li, Z. B. Liang, H. Lin, C. J. Lin, G. L. Lin, S. K. Lin, Y. C. Ling, J. J. Link, J. M. Littenberg, L. Littlejohn, B. R. Liu, D. W. Liu, J. C. Liu, J. L. Liu, Y. B. Lu, C. Lu, H. Q. Luk, A. Luk, K. B. Ma, Q. M. Ma, X. B. Ma, X. Y. Ma, Y. Q. McDonald, K. T. McFarlane, M. C. McKeown, R. D. Meng, Y. Mohapatra, D. Nakajima, Y. Napolitano, J. Naumov, D. Nemchenok, I. Ngai, H. Y. Ngai, W. K. Nie, Y. B. Ning, Z. Ochoa-Ricoux, J. P. Olshevski, A. Patton, S. Pec, V. Peng, J. C. Piilonen, L. E. Pinsky, L. Pun, C. S. J. Qi, F. Z. Qi, M. Qian, X. Raper, N. Ren, J. Rosero, R. Roskovec, B. Ruan, X. C. Shao, B. B. Shih, K. Steiner, H. Sun, G. X. Sun, J. L. Tagg, N. Tam, Y. H. Tanaka, H. K. Tang, X. Themann, H. Torun, Y. Trentalange, S. Tsai, O. Tsang, K. V. Tsang, R. H. M. Tull, C. E. Tung, Y. C. Viren, B. Vorobel, V. Wang, C. H. Wang, L. S. Wang, L. Y. Wang, L. Z. Wang, M. Wang, N. Y. Wang, R. G. Wang, W. Wang, X. Wang, Y. F. Wang, Z. Wang, Z. Wang, Z. M. Webber, D. M. Wei, H. Y. Wei, Y. D. Wen, L. J. Whisnant, K. White, C. G. Whitehead, L. Williamson, Y. Wise, T. Wong, H. L. H. Worcester, E. T. Wu, F. F. Wu, Q. Xi, J. B. Xia, D. M. Xing, Z. Z. Xu, J. Xu, J. Xu, J. L. Xu, Y. Xue, T. Yang, C. G. Yang, L. Ye, M. Yeh, M. Yeh, Y. S. Young, B. L. Yu, Z. Y. Zhan, L. Zhang, C. Zhang, F. H. Zhang, J. W. Zhang, Q. M. Zhang, S. H. Zhang, Y. C. Zhang, Y. H. Zhang, Y. X. Zhang, Z. J. Zhang, Z. P. Zhang, Z. Y. Zhao, J. Zhao, Q. W. Zhao, Y. B. Zheng, L. Zhong, W. L. Zhou, L. Zhou, Z. Y. Zhuang, H. L. Zou, J. H. CA Daya Bay Collaboration TI Improved measurement of electron antineutrino disappearance at Daya Bay SO CHINESE PHYSICS C LA English DT Article DE neutrino oscillation; neutrino mixing; reactor; Daya Bay ID LOADED LIQUID SCINTILLATOR; REACTOR NEUTRINO EXPERIMENT; THETA(13); SPECTRA AB We report an improved measurement of the neutrino mixing angle theta(13) from the Daya Bay Reactor Neutrino Experiment. We exclude a zero value for sin(2)2 theta(13) with a significance of 7.7 standard deviations. Electron antineutrinos from six reactors of 2.9 GW(th) were detected in six antineutrino detectors deployed in two near (flux-weighted baselines of 470 m and 576 m) and one far (1648 m) underground experimental halls. Using 139 days of data, 28909 (205308) electron antineutrino candidates were detected at the far hall (near halls). The ratio of the observed to the expected number of antineutrinos assuming no oscillations at the far hall is 0.944 +/- 0.007(stat.)+/- 0.003(syst.). An analysis of the relative rates in six detectors finds sin(2)2 theta(13)= 0.089 +/- 0.010(stat.)+/- 0.005(syst.) in a three-neutrino framework. C1 [An, F. P.; Bai, J. Z.; Cao, G. F.; Cao, J.; Chang, J. F.; Chen, H. S.; Chen, X. H.; Chen, X. S.; Deng, Z. Y.; Ding, Y. Y.; Du, X. F.; Fu, J. Y.; Guan, M. Y.; He, M.; Heng, Y. K.; Hu, T.; Jetter, S.; Ji, X. L.; Li, F.; Li, Q. J.; Li, W. D.; Li, X. B.; Li, X. N.; Liu, J. C.; Liu, Y. B.; Lu, H. Q.; Ma, Q. M.; Ma, X. Y.; Ma, Y. Q.; Ning, Z.; Qi, F. Z.; Sun, G. X.; Tang, X.; Wang, L. S.; Wang, L. Y.; Wang, R. G.; Wang, Y. F.; Wang, Z. M.; Wen, L. J.; Xia, D. M.; Xing, Z. Z.; Xu, J. L.; Yang, C. G.; Ye, M.; Yu, Z. Y.; Zhan, L.; Zhang, F. H.; Zhang, J. W.; Zhang, S. H.; Zhang, Y. H.; Zhang, Z. Y.; Zhao, J.; Zhao, Q. W.; Zhao, Y. B.; Zhong, W. L.; Zhou, L.; Zhuang, H. L.; Zou, J. H.] Chinese Acad Sci, Inst High Energy Phys, Beijing 100049, Peoples R China. [An, Q.; Hao, H. F.; Liang, H.; Xi, J. B.; Zhang, Y. C.; Zhang, Z. P.; Zheng, L.] Univ Sci & Technol China, Hefei 230026, Peoples R China. [Balantekin, A. B.; Band, H. R.; Cherwinka, J. J.; Heeger, K. M.; Hinrichs, P.; Lewis, C. A.; Littlejohn, B. R.; McFarlane, M. C.; Webber, D. M.; Wise, T.] Univ Wisconsin, Madison, WI USA. [Beriguete, W.; Bishai, M.; Brown, R. L.; Chan, W. T.; Chasman, C.; Diwan, M. V.; Gill, R. L.; Hackenburg, R. W.; Hahn, R. L.; Hans, S.; Issakov, V.; Isvan, Z.; Jaffe, D. E.; Kettell, S. H.; Ling, J. J.; Littenberg, L.; Rosero, R.; Tagg, N.; Tanaka, H. K.; Themann, H.; Viren, B.; Williamson, Y.; Worcester, E. T.; Yeh, M.; Zhang, C.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Blyth, S.; Chang, Y.; Wang, C. H.] Natl United Univ, Miaoli, Taiwan. [Carr, R.; Dwyer, D.; McKeown, R. D.; Qian, X.; Tsang, R. H. M.; Wu, F. F.] CALTECH, Pasadena, CA 91125 USA. [Chen, H. Y.; Hu, B. Z.; Lai, W. H.; Lin, G. L.; Yeh, Y. S.] Natl Chiao Tung Univ, Inst Phys, Hsinchu, Taiwan. [Chen, S. J.; Fang, S. D.; Fu, Z. W.; Qi, M.] Nanjing Univ, Nanjing 210093, Jiangsu, Peoples R China. [Chen, S. M.; Gong, G. H.; Gong, H.; Shao, B. B.; Wang, X.; Wei, H. Y.; Xue, T.] Tsinghua Univ, Dept Engn Phys, Beijing 100084, Peoples R China. [Chen, X. C.; Chu, M. C.; Kwan, K. K.; Kwok, M. W.; Lin, Y. C.; Luk, A.; Shih, K.; Tam, Y. H.] Chinese Univ Hong Kong, Hong Kong, Hong Kong, Peoples R China. [Chen, Y.] Shenzhen Univ, Shenzhen 518060, Peoples R China. [Chen, Y. X.; Ma, X. B.; Wang, L. Z.] N China Elect Power Univ, Beijing 102206, Peoples R China. [Cummings, J. P.] Siena Coll, Loudonville, NY USA. [Draeger, E.; Torun, Y.; White, C. G.] IIT, Dept Phys, Chicago, IL 60616 USA. [Edwards, W. R.; Kramer, M.; Lee, J.; Lin, C. J.; Luk, K. B.; Nakajima, Y.; Ochoa-Ricoux, J. P.; Patton, S.; Steiner, H.; Tsang, K. V.; Tull, C. E.; Wong, H. L. H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Edwards, W. R.; Kramer, M.; Luk, K. B.; Steiner, H.; Wong, H. L. H.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Ely, S. R.; Liu, D. W.; Ngai, W. K.; Peng, J. C.] Univ Illinois, Dept Phys, Urbana, IL USA. [Ge, L. Q.; Jiang, H. J.; Lai, W. C.; Lin, Y. C.] Chengdu Univ Technol, Chengdu 610059, Peoples R China. [Gonchar, M.; Gornushkin, Y. A.; Naumov, D.; Nemchenok, I.; Olshevski, A.] Joint Inst Nucl Res, Dubna, Moscow Region, Russia. [Gu, W. Q.; Li, G. S.; Liu, J. L.] Shanghai Jiao Tong Univ, Shanghai 200240, Peoples R China. [Guo, X. H.; Wang, N. Y.] Beijing Normal Univ, Beijing 100875, Peoples R China. [He, Q.; Lu, C.; McDonald, K. T.] Princeton Univ, Joseph Henry Labs, Princeton, NJ 08544 USA. [Hor, Y. K.; Huber, P.; Link, J. M.; Meng, Y.; Mohapatra, D.; Piilonen, L. E.] Virginia Tech, Ctr Neutrino Phys, Blacksburg, VA USA. [Hsiung, Y. B.; Lai, C. Y.; Tung, Y. C.] Natl Taiwan Univ, Dept Phys, Taipei, Taiwan. [Huang, H. X.; Nie, Y. B.; Ren, J.; Ruan, X. C.; Zhou, Z. Y.] China Inst Atom Energy, Beijing 102413, Peoples R China. [Huang, H. Z.; Trentalange, S.; Tsai, O.] Univ Calif Los Angeles, Los Angeles, CA USA. [Huang, X. T.; Jiao, J. B.; Wang, M.; Wu, Q.] Shandong Univ, Jinan 250100, Peoples R China. [Ji, X. P.; Li, X. Q.; Xu, Y.] Nankai Univ, Sch Phys, Tianjin 300371, Peoples R China. [Johnson, R. A.; Littlejohn, B. R.] Univ Cincinnati, Cincinnati, OH USA. [Kang, L.; Lei, R. T.; Li, Y.; Wei, Y. D.; Yang, L.; Zhang, Z. J.] Dongguan Univ Technol, Dongguan 523808, Peoples R China. [Kwok, T.; Leung, J. K. C.; Leung, K. Y.; Lin, Y. C.; Ngai, H. Y.; Pun, C. S. J.] Univ Hong Kong, Dept Phys, Pokfulam, Hong Kong, Peoples R China. [Lau, K.; Lebanowski, L.; Lin, S. K.; Pinsky, L.; Whitehead, L.] Univ Houston, Dept Phys, Houston, TX USA. [Leitner, R.; Pec, V.; Roskovec, B.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Li, Z. B.] Sun Yat Sen Zhongshan Univ, Guangzhou 510275, Guangdong, Peoples R China. [McKeown, R. D.; Wang, W.] Coll William & Mary, Williamsburg, VA USA. [Napolitano, J.; Raper, N.] Rensselaer Polytech Inst, Troy, NY USA. [Sun, J. L.; Zhang, Y. X.] China Guangdong Nucl Power Grp, Shenzhen 518028, Peoples R China. [Whisnant, K.; Young, B. L.] Iowa State Univ, Ames, IA USA. [Zhang, Q. M.] Xi An Jiao Tong Univ, Xian 710049, Peoples R China. RP An, FP (reprint author), Chinese Acad Sci, Inst High Energy Phys, Beijing 100049, Peoples R China. RI Cao, Jun/G-8701-2012; Wang, Meng/C-4888-2013; Balantekin, Akif Baha/E-4776-2010; Wei, Yen/H-5329-2012; Link, Jonathan/L-2560-2013; Peng, Jun/L-3755-2013; Nemchenok, Igor/F-9715-2014; Wen, Liangjian/C-5113-2015; Olshevskiy, Alexander/I-1580-2016; Ling, Jiajie/I-9173-2014; Liu, Jianglai/P-2587-2015; OI Cao, Jun/0000-0002-3586-2319; Zhong, Weili/0000-0002-4566-5490; HSIUNG, YEE/0000-0003-4801-1238; Qian, Xin/0000-0002-7903-7935; Zhang, Chao/0000-0003-2298-6272; Li, Xiaonan/0000-0003-2857-0219; Torun, Yagmur/0000-0003-2336-6585; Wang, Meng/0000-0003-4067-1127; Balantekin, Akif Baha/0000-0002-2999-0111; Link, Jonathan/0000-0002-1514-0650; Wen, Liangjian/0000-0003-4541-9422; Olshevskiy, Alexander/0000-0002-8902-1793; Ling, Jiajie/0000-0003-2982-0670; Liu, Jianglai/0000-0002-4563-3157; Naumov, Dmitry Vadimovich/0000-0002-0966-8803; Ngai, Ho Yin/0000-0003-0336-2165 FU Ministry of Science and Technology of China; United States Department of Energy; Chinese Academy of Sciences; National Natural Science Foundation of China; Guangdong provincial government; Shenzhen municipal government; China Guangdong Nuclear Power Group; Shanghai Laboratory for Particle Physics and Cosmology; Research Grants Council of the Hong Kong Special Administrative Region of China; University Development Fund of The University of Hong Kong; MOE program for Research of Excellence at NTU; NCTU; NSC fund from Taipei; U.S. National Science Foundation; Alfred P. Sloan Foundation; Ministry of Education, Youth and Sports of the Czech Republic; Czech Science Foundation; Joint Institute of Nuclear Research in Dubna, Russia FX Supported by the Ministry of Science and Technology of China, the United States Department of Energy, the Chinese Academy of Sciences, the National Natural Science Foundation of China, the Guangdong provincial government, the Shenzhen municipal government, the China Guangdong Nuclear Power Group, Shanghai Laboratory for Particle Physics and Cosmology, the Research Grants Council of the Hong Kong Special Administrative Region of China, University Development Fund of The University of Hong Kong, the MOE program for Research of Excellence at NTU, NCTU, and NSC fund support from Taipei, the U.S. National Science Foundation, the Alfred P. Sloan Foundation, the Ministry of Education, Youth and Sports of the Czech Republic, the Czech Science Foundation, and the Joint Institute of Nuclear Research in Dubna, Russia NR 53 TC 190 Z9 192 U1 9 U2 147 PU CHINESE PHYSICAL SOC PI BEIJING PA P O BOX 603, BEIJING 100080, PEOPLES R CHINA SN 1674-1137 J9 CHINESE PHYS C JI Chin. Phys. C PD JAN PY 2013 VL 37 IS 1 AR 011001 DI 10.1088/1674-1137/37/1/011001 PG 20 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA 089EC UT WOS:000314891200001 ER PT J AU Wang, SW Zhang, L Zhang, LL Brinkman, K Chen, FL AF Wang, Siwei Zhang, Lei Zhang, Lingling Brinkman, Kyle Chen, Fanglin TI Two-step sintering of ultrafine-grained barium cerate proton conducting ceramics SO ELECTROCHIMICA ACTA LA English DT Article DE Proton conductor; Co-precipitation; Two-step sintering; Solid oxide fuel cells ID OXIDE FUEL-CELLS; ELECTRICAL-CONDUCTIVITY; ELECTROLYTE; FABRICATION; ZIRCONIA; GROWTH; SOFCS AB Ultra-fine grained dense BaZr0.1Ce0.7Y0.1Yb0.1O3-delta (BZCYYb) ceramics have been successfully prepared via a two-step sintering method. Co-precipitation method has been adopted to prepare nano-sized BZCYYb precursors with an average particle size of 30 nm. By controlling the sintering profile, an average grain size of 184 nm was obtained for dense BZCYYb ceramics via the two-step sintering method, compared to 445 nm for the conventional sintered samples. The two-step sintered BZCYYb samples showed less impurity and an enhanced electrical conductivity compared with the conventional sintered ones. Further, the two-step sintering method was applied to fabricate anode supported solid oxide fuel cells (SOFCs) using BZCYYb as the electrolyte, resulting in dense ultrafine-grained electrolyte membranes and porous anode substrates with fine particles. Due to the reduced ohmic as well as polarization resistances, the maximum power output of the cells fabricated from the two-step sintering method reached 349 mW m(-2) at 700 degrees C, significantly improved from 172 mW cm(-2) for the conventional sintered cells, suggesting that two-step sintering method is very promising for optimizing the microstructure and thus enhancing the electrochemical performances for barium cerate based proton-conducting SOFCs. (C) 2012 Elsevier Ltd. All rights reserved. C1 [Wang, Siwei; Zhang, Lei; Zhang, Lingling; Chen, Fanglin] Univ S Carolina, Dept Mech Engn, Columbia, SC 29208 USA. [Brinkman, Kyle] Savannah River Natl Lab, Aiken, SC 29808 USA. RP Chen, FL (reprint author), Univ S Carolina, Dept Mech Engn, Columbia, SC 29208 USA. EM chenfa@cec.sc.edu RI Wang, Siwei/A-9048-2012; Zhang, Lei/G-8193-2014; Chen, Fanglin/K-1039-2012; OI Chen, Fanglin/0000-0001-9942-8872; zhang, lingling/0000-0001-5038-6915; Wang, Siwei/0000-0001-5118-8267; Brinkman, Kyle/0000-0002-2219-1253 FU DOE Office of Nuclear Energy's Nuclear Energy University Programs FX This research is being performed using funding received from the DOE Office of Nuclear Energy's Nuclear Energy University Programs. NR 29 TC 9 Z9 10 U1 2 U2 42 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0013-4686 J9 ELECTROCHIM ACTA JI Electrochim. Acta PD JAN 1 PY 2013 VL 87 BP 194 EP 200 DI 10.1016/j.electacta.2012.09.007 PG 7 WC Electrochemistry SC Electrochemistry GA 093DE UT WOS:000315171100024 ER PT J AU Ding, JJ Zhou, YN Sun, Q Yu, XQ Yang, XQ Fu, ZW AF Ding, J. J. Zhou, Y. N. Sun, Q. Yu, X. Q. Yang, X. Q. Fu, Z. W. TI Electrochemical properties of P2-phase Na0.74CoO2 compounds as cathode material for rechargeable sodium-ion batteries SO ELECTROCHIMICA ACTA LA English DT Article DE Sodium ion battery; Sodium cobalt oxides; Cathode material ID NA-BATTERIES; ELECTROLYTE; CHALLENGES AB P2-phase Na0.74CoO2 cathode material prepared by a solid-state method exhibits the specific discharge capacity of 107 mAh g(-1) at 0.1 C with good cycling performance for rechargeable sodium ion batteries. The voltage polarization between charging and discharging at 0.1 C rate is about 150-250 mV and the coulombic efficiency in each cycle is about 89%. The expansion and compression in c-axis of the NaxCoO2 unit cell during the Na intercalation/deintercalation is revealed by ex situ XRD. XPS and in situ XAS data directly confirm that deintercalation/intercalation of Na ions from/into the layered structure proceeds with the Co3+/Co4+ redox reaction. (C) 2012 Elsevier Ltd. All rights reserved. C1 [Ding, J. J.; Sun, Q.; Fu, Z. W.] Fudan Univ, Dept Chem & Laser Chem, Shanghai Key Lab Mol Catalysts & Innovat Mat, Shanghai 200433, Peoples R China. [Zhou, Y. N.; Yu, X. Q.; Yang, X. Q.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Fu, ZW (reprint author), Fudan Univ, Dept Chem & Laser Chem, Shanghai Key Lab Mol Catalysts & Innovat Mat, Shanghai 200433, Peoples R China. EM zwfu@fudan.edu.cn RI Sun, Qian/G-4552-2011; Zhou, Yong-Ning/I-9579-2014; Fu, Zheng-wen/I-5880-2016; Yu, Xiqian/B-5574-2014 OI Sun, Qian/0000-0001-5399-1440; Yu, Xiqian/0000-0001-8513-518X FU Science & Technology Commission of Shanghai Municipality [08DZ2270500, 11JC1400500]; 973 Program of China [2011CB933300]; U.S. Department of Energy, the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies [DEAC02-98CH10886] FX This work was financially supported by Science & Technology Commission of Shanghai Municipality (08DZ2270500 and 11JC1400500) and 973 Program (No. 2011CB933300) of China. The work at Brookhaven National Laboratory was supported by the U.S. Department of Energy, the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies, under Contract Number DEAC02-98CH10886. NR 29 TC 53 Z9 54 U1 21 U2 185 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0013-4686 J9 ELECTROCHIM ACTA JI Electrochim. Acta PD JAN 1 PY 2013 VL 87 BP 388 EP 393 DI 10.1016/j.electacta.2012.09.058 PG 6 WC Electrochemistry SC Electrochemistry GA 093DE UT WOS:000315171100051 ER PT J AU Liao, C Sun, XG Dai, S AF Liao, Chen Sun, Xiao-Guang Dai, Sheng TI Crosslinked gel polymer electrolytes based on polyethylene glycol methacrylate and ionic liquid for lithium ion battery applications SO ELECTROCHIMICA ACTA LA English DT Article DE Lithium ion battery; Ionic liquid; Gel polymer electrolyte; LiFePO4; Methylpropylpyrrolidinium bis(trifluoromethanesulfonyl)imdie (MPPY center dot TFSI) ID CONDUCTIVITY; PERFORMANCE; ELECTRODES; FUTURE AB Gel polymer electrolytes were synthesized by copolymerization polyethylene glycol methyl ether methacrylate with polyethylene glycol dimethacrylate in the presence of a room temperature ionic liquid, methylpropylpyrrolidinium bis(trifluoromethanesulfonyl)imide (MPPY center dot TFSI). The physical properties of gel polymer electrolytes were characterized by thermal analysis, impedance spectroscopy, and electrochemical tests. The ionic conductivities of the gel polymer electrolytes increased linearly with the amount of MPPY center dot TFSI and were mainly attributed to the increased ion mobility as evidenced by the decreased glass transition temperatures. Li parallel to LiFePO4 cells were assembled using the gel polymer electrolytes containing 80 wt% MPPY center dot TFSI via an in situ polymerization method. A reversible cell capacity of 90 mAh g(-1) was maintained under the current density of C/10 at room temperature, which was increased to 130 mAh g(-1) by using a thinner membrane and cycling at 50 degrees C. Published by Elsevier Ltd. C1 [Liao, Chen; Sun, Xiao-Guang; Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Dai, Sheng] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. RP Sun, XG (reprint author), Oak Ridge Natl Lab, Div Chem Sci, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. EM sunx@ornl.gov RI liao, chen/E-3755-2012; Dai, Sheng/K-8411-2015 OI liao, chen/0000-0001-5168-6493; Dai, Sheng/0000-0002-8046-3931 FU U.S. Department of Energy's Office of Basic Energy Science, Division of Materials Sciences and Engineering; UT-Battelle, LLC. FX This research was supported by the U.S. Department of Energy's Office of Basic Energy Science, Division of Materials Sciences and Engineering, under contract with UT-Battelle, LLC. NR 33 TC 26 Z9 26 U1 12 U2 101 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0013-4686 J9 ELECTROCHIM ACTA JI Electrochim. Acta PD JAN 1 PY 2013 VL 87 BP 889 EP 894 DI 10.1016/j.electacta.2012.10.027 PG 6 WC Electrochemistry SC Electrochemistry GA 093DE UT WOS:000315171100113 ER PT J AU Nelson, CM Gilmore, TM Harrington, JM Scheckel, KG Miller, BW Bradham, KD AF Nelson, Clay M. Gilmore, Thomas M. Harrington, James M. Scheckel, Kirk G. Miller, Bradley W. Bradham, Karen D. TI Evaluation of a low-cost commercially available extraction device for assessing lead bioaccessibility in contaminated soils SO ENVIRONMENTAL SCIENCE-PROCESSES & IMPACTS LA English DT Article ID RELATIVE BIOAVAILABILITY; RISK-ASSESSMENT; SWINE AB The U.S. EPA's in vitro bioaccessibility (IVBA) method 9200.1-86 defines a validated analytical procedure for the determination of lead bioaccessibility in contaminated soils. The method requires the use of a custom-fabricated extraction device that uses a heated water bath for sample incubation. In an effort to improve ease of use, increase sample throughput, and reduce equipment acquisition and maintenance costs, an alternative low-cost, commercially available extraction device capable of sample incubation via heated air and end-over-end rotation was evaluated. An intra-laboratory study was conducted to compare lead bioaccessibility values derived using the two extraction devices. IVBA values were not statistically different (alpha = 0.05) between the two extraction devices for any of the soils (n = 6) evaluated in this study, with an average difference in mean lead IVBA of 0.8% (s.d. = 0.5%). The commercially available extraction device was able to generate accurate lead IVBA data as compared to the U.S. EPA's expected value for a National Institute of Standards and Technology standard reference material soil. The relative percent differences between high and low IVBA values for each soil, a measure of instrument precision, were also not statistically different (alpha = 0.05) between the two extraction devices. The statistical agreement of lead IVBA values observed using the two extraction devices supports the use of a low-cost, commercially available extraction device as a reliable alternative to a custom-fabricated device as required by EPA method 9200.1-86. C1 [Nelson, Clay M.; Bradham, Karen D.] US EPA, Off Res & Dev, Natl Exposure Res Lab, Durham, NC 27711 USA. [Gilmore, Thomas M.] Natl Caucus & Ctr Black Aged Inc, Senior Environm Employment Program, Durham, NC 27713 USA. [Harrington, James M.; Miller, Bradley W.] Oak Ridge Inst Sci & Educ, Oak Ridge, TN 37831 USA. [Scheckel, Kirk G.] US EPA, Off Res & Dev, Natl Risk Management Res Lab, Cincinnati, OH 45224 USA. RP Nelson, CM (reprint author), US EPA, Off Res & Dev, Natl Exposure Res Lab, Res Triangle Pk,109 TW Alexander Dr,Mail Code D20, Durham, NC 27711 USA. EM nelson.clay@epa.gov RI Scheckel, Kirk/C-3082-2009 OI Scheckel, Kirk/0000-0001-9326-9241 FU United States Environmental Protection Agency through its Office of Research and Development FX The United States Environmental Protection Agency through its Office of Research and Development funded and managed the research described here. It has been subjected to Agency review and approved for publication. Mention of trade names or commercial products does not constitute endorsement or recommendation for use. NR 29 TC 1 Z9 1 U1 0 U2 24 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2050-7887 J9 ENVIRON SCI-PROC IMP JI Environ. Sci.-Process Impacts PY 2013 VL 15 IS 3 BP 573 EP 578 DI 10.1039/c2em30789h PG 6 WC Chemistry, Analytical; Environmental Sciences SC Chemistry; Environmental Sciences & Ecology GA 096IV UT WOS:000315398300004 PM 23738355 ER PT J AU Abraham, DB Maciolek, A AF Abraham, Douglas B. Maciolek, Anna TI Surface states and the Casimir interaction in the Ising model SO EPL LA English DT Article ID VAN-DER-WAALS; TRANSFER-MATRIX; CRITICAL EXPONENTS; CRITICAL-POINT; FORCES; TENSION; MIXTURE; STRIPS; FIELDS AB Using exact calculations, we elucidate the significance of surface states for the Casimir interactions in an Ising strip with a finite width. The surface states are responsible for the strong asymmetry between the super- and sub-critical regimes of the Casimir forces. We introduce an enhanced version of Fisher-Privman theory and justify it using another exact calculation. This gives a rather accurate account of the Casimir scaling function in the sub-critical regime and its exact asymptotic behaviour. We apply analogous ideas in three dimensions and obtain the Casimir scaling function which is in striking agreement with Monte Carlo simulations results for large negative scaling variable. Copyright (C) EPLA, 2013 C1 [Abraham, Douglas B.] Univ Oxford, Dept Phys, Oxford OX1 3NP, England. [Abraham, Douglas B.] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. [Abraham, Douglas B.; Maciolek, Anna] Max Planck Inst Intelligente Systeme, D-70569 Stuttgart, Germany. [Maciolek, Anna] Univ Stuttgart, Inst Theoret Phys 4, D-70569 Stuttgart, Germany. [Maciolek, Anna] Polish Acad Sci, Inst Phys Chem, Dept 3, PL-01224 Warsaw, Poland. RP Abraham, DB (reprint author), Univ Oxford, Dept Phys, 1 Keble Rd, Oxford OX1 3NP, England. FU Center for Non-linear Studies at Los Alamos National Lab FX DBA acknowledges the support of Prof. S. Dietrich at the MPI Stuttgart and of the Center for Non-linear Studies at Los Alamos National Lab, where parts of this work were done. NR 39 TC 9 Z9 9 U1 0 U2 6 PU EPL ASSOCIATION, EUROPEAN PHYSICAL SOCIETY PI MULHOUSE PA 6 RUE DES FRERES LUMIERE, MULHOUSE, 68200, FRANCE SN 0295-5075 J9 EPL-EUROPHYS LETT JI EPL PD JAN PY 2013 VL 101 IS 2 AR 20006 DI 10.1209/0295-5075/101/20006 PG 6 WC Physics, Multidisciplinary SC Physics GA 086IK UT WOS:000314677100006 ER PT J AU Lewicki, JP Albo, RLF Alviso, CT Maxwell, RS AF Lewicki, James P. Albo, Rebecca L. F. Alviso, Cynthia T. Maxwell, Robert S. TI Pyrolysis-gas chromatography/mass spectrometry for the forensic fingerprinting of silicone engineering elastomers SO JOURNAL OF ANALYTICAL AND APPLIED PYROLYSIS LA English DT Article DE Poly (dimethylsiloxane); Multivariate analysis; Silicone elastomers; Thermal degradation ID INDUCED CROSS-LINKING; THERMAL-DEGRADATION; MECHANICAL-PROPERTIES; POLYSILOXANE RUBBERS; MQ-NMR; NETWORKS; RADIATION; MODEL; POLY(DIMETHYLSILOXANE); PRECIPITATION AB In this study, pyrolysis gas chromatography paired with mass spectrometry (Py-GC/MS) has been investigated as an analytical technique for the identification and discrimination of commercial silicone elastomer formulations. Multivariate statistical analysis, specifically principle component analysis (PCA), was utilized in order to provide a direct link between the fingerprint behavior and the starting network structure. This work utilizes PCA to "map" the pyrolysis analyses such that underlying chemistries, systematic similarities, fillers, and morphologies may be predicted. It has been demonstrated that silicone materials formulated via differing cure chemistries have distinct degradation fingerprints. The application of PCA statistical methodologies to Py-GC/MS data allows these unique signatures to be rapidly and reliably identified. Furthermore, PCA allows the chemical origins of the degradation fingerprints to be assessed with comparative ease. (c) 2012 Elsevier B.V. All rights reserved. C1 [Lewicki, James P.; Albo, Rebecca L. F.; Alviso, Cynthia T.; Maxwell, Robert S.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Lewicki, JP (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. EM lewicki1@llnl.gov FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 22 TC 3 Z9 3 U1 2 U2 39 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0165-2370 J9 J ANAL APPL PYROL JI J. Anal. Appl. Pyrolysis PD JAN PY 2013 VL 99 BP 85 EP 91 DI 10.1016/j.jaap.2012.10.021 PG 7 WC Chemistry, Analytical; Spectroscopy SC Chemistry; Spectroscopy GA 094CN UT WOS:000315240700012 ER PT J AU Dees, DW Gallagher, KG Abraham, DP Jansen, AN AF Dees, Dennis W. Gallagher, Kevin G. Abraham, Daniel P. Jansen, Andrew N. TI Electrochemical Modeling the Impedance of a Lithium-Ion Positive Electrode Single Particle SO JOURNAL OF THE ELECTROCHEMICAL SOCIETY LA English DT Article ID 3-DIMENSIONAL MICROSTRUCTURE; INSERTION CELL; BATTERY; LINI0.8CO0.15AL0.05O2; OPTIMIZATION AB A three-dimensional electrochemical model was developed to examine the performance (i.e. impedance determined by a pulse change in potential) of a lithium-ion intercalation positive electrode single particle. A comprehensive parameter study was conducted, based on a layered nickel oxide parameter set previously developed. The dominance of the interfacial impedance on the particle performance accentuates the impact of the secondary particle porosity and electrolyte wetting of the porosity. Electronic distribution effects, including conductivity and particle contacts, also become significant when the secondary particle's effective conductivity is less than about 10(-5) Omega(-1) cm(-1). Most of the simulations were conducted using a spherical shaped secondary particle, but other spheroidal geometries are considered, which only has a marginal impact on particle impedance. (C) 2013 The Electrochemical Society. [DOI: 10.1149/2.055303jes] All rights reserved. C1 [Dees, Dennis W.; Gallagher, Kevin G.; Abraham, Daniel P.; Jansen, Andrew N.] Argonne Natl Lab, Chem Sci & Engn Div, Electrochem Energy Storage, Argonne, IL 60439 USA. RP Dees, DW (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, Electrochem Energy Storage, 9700 S Cass Ave, Argonne, IL 60439 USA. EM dees@anl.gov RI Jansen, Andrew/Q-5912-2016 OI Jansen, Andrew/0000-0003-3244-7790 FU U.S. Department of Energy Office of Science laboratory [DE-AC02-06CH11357]; Vehicle Technologies Program, Hybrid and Electric Systems FX Support from the Vehicle Technologies Program, Hybrid and Electric Systems, David Howell (Team Lead) and Peter Faguy, at the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, is gratefully acknowledged. The submitted manuscript has been created by UChicago Argonne, LLC, Operator of Argonne National Laboratory ("Argonne"). Argonne, a U.S. Department of Energy Office of Science laboratory, is operated under Contract No. DE-AC02-06CH11357. The U.S. Government retains for itself, and others acting on its behalf, a paid-up nonexclusive, irrevocable worldwide license in said article to reproduce, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, by or on behalf of the Government. NR 29 TC 7 Z9 7 U1 5 U2 72 PU ELECTROCHEMICAL SOC INC PI PENNINGTON PA 65 SOUTH MAIN STREET, PENNINGTON, NJ 08534 USA SN 0013-4651 J9 J ELECTROCHEM SOC JI J. Electrochem. Soc. PY 2013 VL 160 IS 3 BP A478 EP A486 DI 10.1149/2.055303jes PG 9 WC Electrochemistry; Materials Science, Coatings & Films SC Electrochemistry; Materials Science GA 095AS UT WOS:000315307500011 ER PT J AU Deng, J Wagner, GJ Muller, RP AF Deng, Jie Wagner, Gregory J. Muller, Richard P. TI Phase Field Modeling of Solid Electrolyte Interface Formation in Lithium Ion Batteries SO JOURNAL OF THE ELECTROCHEMICAL SOCIETY LA English DT Article ID LI-ION; GRAPHITE-ELECTRODES; SURFACE-CHEMISTRY; RECHARGEABLE BATTERIES; LIFEPO4 NANOPARTICLES; ETHYLENE CARBONATE; THERMAL-STABILITY; INTERPHASE; MECHANISMS; ANODES AB A phase field model is presented to capture the formation of a solid electrolyte interface (SEI) layer on the anode surface in lithium ion batteries. In this model, the formation of an SET layer is treated as a phase transformation process where the electrolyte phase is transformed to the SEI phase due to electrochemical reactions at the SEI/electrolyte interface during SEI growth. Numerical results show that SEI growth exhibits a power-law scaling with respect to time and is limited by the diffusion of electrons across the SET layer. It is found that during SET growth,. the gradients of both electric potential and concentrations of species are built inside of the SEI layer, and the charge separation at the SEI/electrolyte interface remains with decreasing charge density at the interfacial region. The effects of various factors such as initial conditions, electron diffusivity, SET formation rate, applied current density and temperature on the SEI growth rate and the distribution of electric potential and concentrations of species are investigated. The capabilities of the present model and its extension are also discussed. (C) 2013 The ElectroChemical Society. [DOT: 10.1149/2.052303jes] All rights reserved. C1 [Deng, Jie; Wagner, Gregory J.] Sandia Natl Labs, Thermal Fluid Sci & Engn Dept, Livermore, CA 94550 USA. [Muller, Richard P.] Sandia Natl Labs, Adv Device Technol Dept, Albuquerque, NM 87185 USA. RP Deng, J (reprint author), Sandia Natl Labs, Thermal Fluid Sci & Engn Dept, Livermore, CA 94550 USA. EM jd04e@my.fsu.edu RI Wagner, Gregory/I-4377-2015 FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Authors appreciate discussions with Dr. Jonathan E. Guyer at the National Institute of Standards and Technology. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 48 TC 16 Z9 17 U1 5 U2 110 PU ELECTROCHEMICAL SOC INC PI PENNINGTON PA 65 SOUTH MAIN STREET, PENNINGTON, NJ 08534 USA SN 0013-4651 J9 J ELECTROCHEM SOC JI J. Electrochem. Soc. PY 2013 VL 160 IS 3 BP A487 EP A496 DI 10.1149/2.052303jes PG 10 WC Electrochemistry; Materials Science, Coatings & Films SC Electrochemistry; Materials Science GA 095AS UT WOS:000315307500012 ER PT J AU Hallinan, DT Mullin, SA Stone, GM Balsara, NP AF Hallinan, Daniel T. Mullin, Scott A. Stone, Gregory M. Balsara, Nitash P. TI Lithium Metal Stability in Batteries with Block Copolymer Electrolytes SO JOURNAL OF THE ELECTROCHEMICAL SOCIETY LA English DT Article ID POLYMER ELECTROLYTES; RECHARGEABLE BATTERIES; MOLECULAR-WEIGHT; CONDUCTIVITY; CELLS; BEHAVIOR; TEMPERATURE; LIMITATIONS; SPECTRA; GROWTH AB Lithium dendrite formation was studied in polymer electrolytes consisting of lithium bis(trifluoromethanesulfonyl)imide salt (LiTFSI) dissolved in polystyrene-b-poly(ethylene oxide) block copolymers. Both Li-polymer-FePO4 batteries and Li-polymer-Li symmetric cells were cycled at constant current until voltage responses characteristic of dendritic failure were observed. The amount of charge passed before this observation was defined as the lifetime of the cell. Battery lifetimes were found to be significantly longer than symmetric cell lifetimes. Both battery and symmetric cell lifetimes increased with increasing electrolyte thickness, as predicted by the model of Monroe and Newman. Post-mortem analysis of the lithium surfaces were conducted after failure. The lithium electrodes from failed batteries were much smoother than those from failed symmetric cells. Dendritic structures with characteristic length scales in the 10-30 mu m range were seen in batteries. In contrast, the length scales of the dendritic structures seen in symmetric cells were in the 100-300 mu m range. (C) 2013 The Electrochemical Society. [DOI: 10.1149/2.030303jes] All rights reserved. C1 [Hallinan, Daniel T.; Mullin, Scott A.; Balsara, Nitash P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Mullin, Scott A.; Stone, Gregory M.; Balsara, Nitash P.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Stone, Gregory M.; Balsara, Nitash P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Hallinan, DT (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. EM nbalsara1@gmail.com FU Office of Vehicle Technologies of the U.S. Department of Energy [DE-AC02-05CH11231] FX The authors thank Professor John Newman for numerous helpful discussions, and for the use of his Maccor cycler and convection ovens. This work was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 43 TC 35 Z9 35 U1 14 U2 139 PU ELECTROCHEMICAL SOC INC PI PENNINGTON PA 65 SOUTH MAIN STREET, PENNINGTON, NJ 08534 USA SN 0013-4651 J9 J ELECTROCHEM SOC JI J. Electrochem. Soc. PY 2013 VL 160 IS 3 BP A464 EP A470 DI 10.1149/2.030303jes PG 7 WC Electrochemistry; Materials Science, Coatings & Films SC Electrochemistry; Materials Science GA 095AS UT WOS:000315307500009 ER PT J AU Xiang, B Wang, L Liu, G Minor, AM AF Xiang, Bin Wang, Lei Liu, Gao Minor, Andrew M. TI Electromechanical Probing of Li/Li2CO3 Core/Shell Particles in a TEM SO JOURNAL OF THE ELECTROCHEMICAL SOCIETY LA English DT Article ID LITHIUM-CARBONATE; BATTERIES; CHALLENGES AB We provide a detailed electromechanical study of individual core/shell structure - Li metal/Li2CO3 particles by utilizing an in-situ probing technique in the transmission electron microscope (TEM). This technique allows us to concurrently monitor the mechanical and electrical response of single Li/Li2CO3 core/shell structures in real time. The pressure on the Li/Li2CO3 core/shell particle was measured to be similar to 15 MPa at the initiation of fracture and the conductivity of the Li2CO3 shell is estimated to be similar to 10(-6) S/cm. To simulate the application of the core-shell particles in a real battery, we assembled coin cells with Li metal as a counter electrode. Prior to the cell assembly, the electrode was compressed in order to break the Li2CO3 shells to expose the fresh lithium metal to the graphite. When the electrolyte is added to wet the electrode, an electrochemical reaction spontaneously occurs between the exposed Li and graphite particles to produce a partially lithiated graphite anode. This lithiation occurs prior to the initial charging process, therefore compensating for the irreversible capacity loss due to the lithium consummation events during standard formation.(1-3) Our results demonstrate a new pathway for the utilization of non-lithiated cathode material in future Li-ion batteries. (C) 2013 The Electrochemical Society. [DOI: 10.1149/2.018303jes] All rights reserved. C1 [Xiang, Bin; Minor, Andrew M.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Xiang, Bin; Minor, Andrew M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Natl Ctr Electron Microscopy, Berkeley, CA 94720 USA. [Wang, Lei; Liu, Gao] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. RP Xiang, B (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. EM gliu@lbl.gov; aminor@lbl.gov RI Wang, Lei/D-4773-2012; Xiang, Bin/C-9192-2012; Foundry, Molecular/G-9968-2014 FU Office of Vehicle Technologies of the U.S. Department of Energy under the Batteries for Advanced Transportation Technologies (BATT) Program [DE-AC02-05CH11231]; Office of Vehicle Technologies of the U.S. Department of Energy under the Integrated Laboratory/Industry Research Program (IRLIP) [DE-AC02-05CH11231]; National Center for Electron Microscopy, Lawrence Berkeley Lab by U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231, under the Batteries for Advanced Transportation Technologies (BATT) Program and the Integrated Laboratory/Industry Research Program (IRLIP). The Stabilized Lithium Metal Powder (SLMP) was supplied by FMC Lithium Corp.. The authors acknowledge support of the National Center for Electron Microscopy, Lawrence Berkeley Lab, which is supported by the U.S. Department of Energy under Contract # DE-AC02-05CH11231. NR 15 TC 7 Z9 8 U1 4 U2 50 PU ELECTROCHEMICAL SOC INC PI PENNINGTON PA 65 SOUTH MAIN STREET, PENNINGTON, NJ 08534 USA SN 0013-4651 J9 J ELECTROCHEM SOC JI J. Electrochem. Soc. PY 2013 VL 160 IS 3 BP A415 EP A419 DI 10.1149/2.018303jes PG 5 WC Electrochemistry; Materials Science, Coatings & Films SC Electrochemistry; Materials Science GA 095AS UT WOS:000315307500001 ER PT J AU Small, L Brumbach, M Apblett, C Ihlefeld, JF Brennecka, G Duquette, D AF Small, Leo Brumbach, Michael Apblett, Christopher Ihlefeld, Jon F. Brennecka, Geoff Duquette, David TI On the Degradation Processes of Thin Film PZT in 0.1 N H2SO4 SO JOURNAL OF THE ELECTROCHEMICAL SOCIETY LA English DT Article ID ANODIC PASSIVE FILMS; X-RAY PHOTOELECTRON; POINT-DEFECT MODEL; WET BALL-MILL; IMPEDANCE SPECTROSCOPY; ZIRCONIUM-PHOSPHATE; SULFATED-ZIRCONIA; CHEMICAL-STATE; LEAD; OXIDATION AB Electrochemical impedance spectroscopy is used to monitor the real-time network response of 1 cm(2) areas of ferroelectric PbZr0.52Ti0.48O3 (PZT) thin films solution deposited onto platinized silicon wafers and exposed to 0.1 N H2SO4 over 48 hours. Development of equivalent circuits to model the competing processes of pore growth, interfacial layer formation, and uniform chemical attack are guided by the evolution of film structure and chemistry as observed ex-situ in SEM, X-ray photoelectron spectroscopy, and X-ray diffraction. In areas containing cracks or pores, corrosion is accelerated. After prolonged exposure, growth of an amorphous film of PbSO4, sulfate-doped zirconia, and lead-deficient PZT proceeds into the PZT film, with PbSO4 crystals nucleating atop this interfacial layer. The Point Defect Model for the passive state is used to explain the dissolution processes observed in the complex oxide. Application of this model to PbZrxTi1-xO3 for x = 0.25, 0.52, and 0.95 points to the role of titanium in the creation of an ionically insulating layer that impedes further chemical attack. (C) 2013 The Electrochemical Society. [DOT: 10.1149/2.005304jes] All rights reserved. C1 [Small, Leo; Duquette, David] Rensselaer Polytech Inst, Dept Mat Sci & Engn, Troy, NY 12180 USA. [Small, Leo; Brumbach, Michael; Apblett, Christopher; Ihlefeld, Jon F.; Brennecka, Geoff] Sandia Natl Labs, Albuquerque, NM 87105 USA. RP Small, L (reprint author), Rensselaer Polytech Inst, Dept Mat Sci & Engn, Troy, NY 12180 USA. EM ljsmall@sandia.gov RI Small, Leo/A-3685-2013; Ihlefeld, Jon/B-3117-2009; Brennecka, Geoff/J-9367-2012 OI Small, Leo/0000-0003-0404-6287; Brennecka, Geoff/0000-0002-4476-7655 FU Laboratory Directed Research and Development (LDRD) program; National Institute of Nano Engineering (NINE) at Sandia National Laboratories; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors thank Bonnie B. McKenzie for help acquiring SEM images. This work was supported by the Laboratory Directed Research and Development (LDRD) program and the National Institute of Nano Engineering (NINE) at Sandia National Laboratories. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 53 TC 0 Z9 0 U1 0 U2 16 PU ELECTROCHEMICAL SOC INC PI PENNINGTON PA 65 SOUTH MAIN STREET, PENNINGTON, NJ 08534 USA SN 0013-4651 J9 J ELECTROCHEM SOC JI J. Electrochem. Soc. PY 2013 VL 160 IS 3 BP C128 EP C135 DI 10.1149/2.005304jes PG 8 WC Electrochemistry; Materials Science, Coatings & Films SC Electrochemistry; Materials Science GA 095AS UT WOS:000315307500026 ER PT J AU Tian, D Li, N Xiao, N Wang, FF Yu, SY Li, Q Gao, W Wu, G AF Tian, Dong Li, Ning Xiao, Ning Wang, Fang F. Yu, Shi Y. Li, Qing Gao, Wei Wu, Gang TI Replacement Deposition of Ni-S Films on Cu and Their Catalytic Activity for Electroless Nickel Plating SO JOURNAL OF THE ELECTROCHEMICAL SOCIETY LA English DT Article ID FUNCTIONAL THEORY ANALYSIS; HYPOPHOSPHITE IONS; METAL-SURFACES; THIN-FILMS; COPPER; THIOUREA; SULFUR; ACTIVATION; OXIDATION; XPS AB A Ni-S film was prepared on Cu substrate via the replacement reaction due to the quite negative electrode potential of Cu in high concentrated thiourea solution. A lower pH environment was facilitated to form more uniform Ni-S film. The sulfur content in the Ni-S film increased with the increase of deposition time and the rise of pH in solution. Relative to pure Ni, the existence of sulfur in the Ni-S film was found to result in different electrochemical properties. More importantly, constant current discharge curve and anodic polarization curve measurements indicated that the Ni-S film with higher sulfur content was more prone to be passivated, with negative influences on its catalytic activity. Polarization curve, electrochemical impedance spectroscopy and open circuit potential measurements were employed to investigate the catalytic activity of the Ni-S film for hypophosphite oxidation and electroless nickel (EN) plating. With the optimization of sulfur content by plating conditions, we could significantly improve the catalytic activity of the Ni-S film for hypophosphite oxidation and consequently for EN plating. Compared with the traditional Pd film, the Ni-S film exhibited a comparable catalytic activity, with a uniform electroless Ni-P layer obtained during the EN plating. (C) 2013 The Electrochemical Society. [DOI: 10.1149/2.034303jes] All rights reserved. C1 [Tian, Dong; Li, Ning; Xiao, Ning; Yu, Shi Y.] Harbin Inst Technol, Sch Chem Engn & Technol, Harbin 150001, Peoples R China. [Wang, Fang F.] Xiamen Univ, Coll Chem & Chem Engn, Dept Chem, Xiamen 361005, Peoples R China. [Li, Qing; Gao, Wei; Wu, Gang] Los Alamos Natl Lab, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA. RP Tian, D (reprint author), Harbin Inst Technol, Sch Chem Engn & Technol, Harbin 150001, Peoples R China. EM lininghit@263.net RI Wu, Gang/E-8536-2010; Li, Qing/G-4502-2011 OI Wu, Gang/0000-0003-4956-5208; Li, Qing/0000-0003-4807-030X FU Highnic Group FX The financial support by Highnic Group in this work is gratefully acknowledged. NR 46 TC 4 Z9 4 U1 3 U2 42 PU ELECTROCHEMICAL SOC INC PI PENNINGTON PA 65 SOUTH MAIN STREET, PENNINGTON, NJ 08534 USA SN 0013-4651 J9 J ELECTROCHEM SOC JI J. Electrochem. Soc. PY 2013 VL 160 IS 3 BP D95 EP D101 DI 10.1149/2.034303jes PG 7 WC Electrochemistry; Materials Science, Coatings & Films SC Electrochemistry; Materials Science GA 095AS UT WOS:000315307500032 ER PT J AU Wixtrom, AI Buhler, JE Reece, CE Abdel-Fattah, TM AF Wixtrom, Alex I. Buhler, Jessica E. Reece, Charles E. Abdel-Fattah, Tarek M. TI Electrochemical Polishing Applications and EIS of a Vitamin B-4-Based Ionic Liquid SO JOURNAL OF THE ELECTROCHEMICAL SOCIETY LA English DT Article ID NIOBIUM AB Modem particle accelerators require minimal interior surface roughness for Niobium superconducting radio frequency (SRF) cavities. Polishing of the Nb is currently achieved via electrochemical polishing with concentrated mixtures of sulfuric and hydrofluoric acids. This acid-based approach is effective at reducing the surface roughness to acceptable levels for SRF use, but due to acid-related hazards and extra costs (including safe disposal of used polishing solutions), an acid-free method would be preferable. This study focuses on an alternative electrochemical polishing method for Nb, using a novel ionic liquid solution containing choline chloride, also known as Vitamin B-4 (VB4). Potentiostatic electrochemical impedance spectroscopy (EIS) was also performed on the VB4-based system. Nb polished using the VB4-based method was found to have a final surface roughness comparable to that achieved via the acid-based method, as assessed by atomic force microscopy (AFM). These findings indicate that acid-free VB4-based electrochemical polishing of Nb represents a promising replacement for acid-based methods of SRF cavity preparation. (C) 2013 The Electrochemical Society. [DOI: 10.1149/2.013303jes] All rights reserved. C1 [Wixtrom, Alex I.; Buhler, Jessica E.; Abdel-Fattah, Tarek M.] Christopher Newport Univ, Thomas Jefferson Natl Accelerator Facil, Appl Res Ctr, Newport News, VA 23606 USA. [Wixtrom, Alex I.; Buhler, Jessica E.; Abdel-Fattah, Tarek M.] Christopher Newport Univ, Dept Mol Biol & Chem, Newport News, VA 23606 USA. [Reece, Charles E.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. RP Wixtrom, AI (reprint author), Christopher Newport Univ, Thomas Jefferson Natl Accelerator Facil, Appl Res Ctr, Newport News, VA 23606 USA. EM fattah@cnu.edu FU NSF [0959807] FX This research was conducted at Thomas Jefferson National Accelerator Facility and Christopher Newport University, Department of Molecular Biology and Chemistry. We would also like to acknowledge the Surface Characterization Lab of College of William and Mary at Applied Research Center - Jefferson Labs, Newport News for the use of their characterization equipment. The authors gratefully acknowledge the financial support from NSF award no. 0959807. NR 12 TC 2 Z9 2 U1 0 U2 14 PU ELECTROCHEMICAL SOC INC PI PENNINGTON PA 65 SOUTH MAIN STREET, PENNINGTON, NJ 08534 USA SN 0013-4651 EI 1945-7111 J9 J ELECTROCHEM SOC JI J. Electrochem. Soc. PY 2013 VL 160 IS 3 BP E22 EP E26 DI 10.1149/2.013303jes PG 5 WC Electrochemistry; Materials Science, Coatings & Films SC Electrochemistry; Materials Science GA 095AS UT WOS:000315307500038 ER PT J AU Wang, X Ahluwalia, RK Steinbach, AJ AF Wang, X. Ahluwalia, R. K. Steinbach, A. J. TI Kinetics of Hydrogen Oxidation and Hydrogen Evolution Reactions on Nanostructured Thin-Film Platinum Alloy Catalyst SO JOURNAL OF THE ELECTROCHEMICAL SOCIETY LA English DT Article ID OXYGEN REDUCTION REACTION; FUEL-CELLS; CO; PERFORMANCE; ACID AB Kinetics of hydrogen oxidation (HOR) and hydrogen evolution (HER) reactions on nanostructured thin-film (NSTF) ternary Pt0.68Co0.3Mn0.02 catalyst was investigated in a 50-cm(2) polymer electrolyte fuel cell operated in H-2 pump mode with super-saturated feeds, at 45-90 degrees C and 0.7-2.5 atm H-2 partial pressures. The results showed that the HOR and HER are completely reversible, and that both of these reactions can be described by the same Butler-Volmer kinetics with first-order dependence on the H-2 partial pressure. The specific exchange current density for the 2-electron HOR/HER on the NSTF ternary catalyst, derived from the measured polarization curves, is 489 mA.cm(Pt)(-2) at 80 degrees C and 1-atm H-2 partial pressure. The temperature dependence of the exchange current density is consistent with an activation energy of 38.9 kJ.mol(-1). Compared to dispersed Pt/C catalyst with an ultralow 0.003 mg.cm(-2) Pt loading, the HOR kinetics on NSTF catalyst with 0.05-0.10 mg.cm(-2) Pt loading was 60-110% faster on an area-specific basis, but it was slower on a mass basis. The measured HOR/HER kinetics is a function of the state of the catalyst in that the specific exchange current density increased by 460% when the anode catalyst was conditioned with the same protocol normally used for the cathode catalyst. (C) 2013 The Electrochemical Society. [DOT: 10.1149/2.028303jes] All rights reserved. C1 [Wang, X.; Ahluwalia, R. K.] Argonne Natl Lab, Argonne, IL 60439 USA. [Steinbach, A. J.] 3M Fuel Cell Components Program, St Paul, MN 55144 USA. RP Wang, X (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. EM x.wang@anl.gov FU Office of Fuel Cell Technologies of the U.S. Department of Energy's Office of Energy Efficiency and Renewable Energy FX This work was supported by the Office of Fuel Cell Technologies of the U.S. Department of Energy's Office of Energy Efficiency and Renewable Energy. Dr. Nancy Garland and Jason Marcinkoski were the DOE program managers for this work. NR 21 TC 11 Z9 11 U1 3 U2 68 PU ELECTROCHEMICAL SOC INC PI PENNINGTON PA 65 SOUTH MAIN STREET, PENNINGTON, NJ 08534 USA SN 0013-4651 J9 J ELECTROCHEM SOC JI J. Electrochem. Soc. PY 2013 VL 160 IS 3 BP F251 EP F261 DI 10.1149/2.028303jes PG 11 WC Electrochemistry; Materials Science, Coatings & Films SC Electrochemistry; Materials Science GA 095AS UT WOS:000315307500042 ER PT J AU Wu, QH Ok, JT Sun, YP Retterer, ST Neeves, KB Yin, XL Bai, BJ Ma, YF AF Wu, Qihua Ok, Jeong Tae Sun, Yongpeng Retterer, S. T. Neeves, Keith B. Yin, Xiaolong Bai, Baojun Ma, Yinfa TI Optic imaging of single and two-phase pressure-driven flows in nano-scale channels dagger SO LAB ON A CHIP LA English DT Article ID MICROFLUIDIC DEVICES; DRUG-DELIVERY; VOID FRACTION; NANOCHANNELS; DROP; MICROCHANNELS; FABRICATION; DISPERSION; DYNAMICS; PATTERN AB Microfluidic and nanofluidic devices have undergone rapid development in recent years. Functions integrated onto such devices provide lab-on-a-chip solutions for many biomedical, chemical, and engineering applications. In this paper, a lab-on-a-chip technique for direct visualization of the single- and two-phase pressure-driven flows in nano-scale channels was developed. The nanofluidic chip was designed and fabricated; concentration dependent fluorescence signal correlation was developed for the determination of flow rate. Experiments of single and two-phase flow in nano-scale channels with 100 nm depth were conducted. The linearity correlation between flow rate and pressure drop in nanochannels was obtained and fit closely into Poiseuille's Law. Meanwhile, three different flow patterns, single, annular, and stratified, were observed from the two-phase flow in the nanochannel experiments and their special features were described. A two-phase flow regime map for nanochannels is presented. Results are of critical importance to both fundamental study and many applications. C1 [Wu, Qihua; Ma, Yinfa] Missouri Univ Sci & Technol, Dept Chem, Rolla, MO USA. [Ok, Jeong Tae; Neeves, Keith B.] Colorado Sch Mines, Dept Chem & Biol Engn, Golden, CO 80401 USA. [Sun, Yongpeng; Bai, Baojun] Missouri Univ Sci & Technol, Dept Petr Engn, Rolla, MO USA. [Retterer, S. T.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci Div, Oak Ridge, TN USA. [Yin, Xiaolong] Colorado Sch Mines, Dept Petr Engn, Golden, CO 80401 USA. RP Bai, BJ (reprint author), Missouri Univ Sci & Technol, Dept Petr Engn, Rolla, MO USA. EM baib@mst.edu; yinfa@mst.edu RI Retterer, Scott/A-5256-2011; Wu, Qihua/K-2541-2015 OI Retterer, Scott/0000-0001-8534-1979; Wu, Qihua/0000-0002-2243-936X FU Ultra-Deep water and Unconventional Natural Gas and Other Petroleum Resources program FX Funding for this project is provided by the Research Partnership to Secure Energy for America (RPSEA) through the Ultra-Deep water and Unconventional Natural Gas and Other Petroleum Resources program authorized by the US Energy Policy Act of 2005. A portion of this research was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Office of Basic Energy Sciences, U.S. Department of Energy. The authors acknowledge the help of Professor Ralph Jimenez and Jennifer Lubbeck in the Department of Chemistry & Biochemistry at the University of Colorado, Boulder for assistance with anodic bonding. NR 39 TC 12 Z9 12 U1 4 U2 40 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1473-0197 J9 LAB CHIP JI Lab Chip PY 2013 VL 13 IS 6 BP 1165 EP 1171 DI 10.1039/c2lc41259d PG 7 WC Biochemical Research Methods; Chemistry, Multidisciplinary; Nanoscience & Nanotechnology SC Biochemistry & Molecular Biology; Chemistry; Science & Technology - Other Topics GA 093BL UT WOS:000315166600023 PM 23370894 ER PT J AU Chandrakumar, KRS Readle, JD Rouleau, C Puretzky, A Geohegan, DB More, K Krishnan, V Tian, MK Duscher, G Sumpter, B Irle, S Morokuma, K AF Chandrakumar, K. R. S. Readle, Jason D. Rouleau, Chris Puretzky, Alex Geohegan, David B. More, Karren Krishnan, Veena Tian, Mengkun Duscher, Gerd Sumpter, Bobby Irle, Stephan Morokuma, Keiji TI High-temperature transformation of Fe-decorated single-wall carbon nanohorns to nanooysters: a combined experimental and theoretical study SO NANOSCALE LA English DT Article ID LASER VAPORIZATION; MOLECULAR-DYNAMICS; GRAPHITIC CONES; CONDENSED-PHASE; AB-INITIO; NANOTUBES; GROWTH; GRAPHENE; NUCLEATION; SIMULATIONS AB The processes by which single-wall carbon nanohorns are transformed by iron nanoparticles at high temperatures to form "nanooysters", hollow graphene capsules containing metal particles that resemble pearls in an oyster shell, are examined both experimentally and theoretically. Quantum chemical molecular dynamics (QM/MD) simulations based on the density-functional tight-binding (DFTB) method were performed to investigate their growth mechanism. The simulations suggest that the nanoparticles self-encapsulate to form single-wall nanooysters (SWNOs) by assisting the assembly of dangling carbon bonds, accompanied by migration of the metal particle inside the carbon structure. These calculations indicate that the structure of the oyster consists primarily of hexagons along with a few pentagons that are predominantly formed near the former nanohorn edges as a result of their fusion. Experimental observations of large diameter nanoparticles inside multiwall carbon shells indicate that migration and coalescence of many iron particles must occur, perhaps by the convergence of smaller SWNOs or carbon-coated Fe-nanoparticles, whereby the void space is generated by the corresponding increase in the carbon shell surface area to metal nanoparticle volume. C1 [Chandrakumar, K. R. S.; Morokuma, Keiji] Kyoto Univ, Fukui Inst Fundamental Chem, Kyoto 6068103, Japan. [Irle, Stephan] Nagoya Univ, Inst Adv Res, Nagoya, Aichi 4648602, Japan. [Irle, Stephan] Nagoya Univ, Dept Chem, Nagoya, Aichi 4648602, Japan. [Readle, Jason D.; Rouleau, Chris; Puretzky, Alex; Geohegan, David B.; More, Karren; Duscher, Gerd; Sumpter, Bobby] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Krishnan, Veena; Tian, Mengkun; Duscher, Gerd] Univ Tennessee, Knoxville, TN USA. RP Geohegan, DB (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. EM geohegandb@ornl.gov; sirle@chem.nagoya-u.ac.jp; keiji.morokuma@emory.edu RI Chandrakumar, KRS/G-2478-2010; Sumpter, Bobby/C-9459-2013; Geohegan, David/D-3599-2013; Duscher, Gerd/G-1730-2014; Rouleau, Christopher/Q-2737-2015; More, Karren/A-8097-2016; Puretzky, Alexander/B-5567-2016; Irle, Stephan/E-8984-2011 OI Chandrakumar, KRS/0000-0002-0121-3556; Sumpter, Bobby/0000-0001-6341-0355; Geohegan, David/0000-0003-0273-3139; Duscher, Gerd/0000-0002-2039-548X; Rouleau, Christopher/0000-0002-5488-3537; More, Karren/0000-0001-5223-9097; Puretzky, Alexander/0000-0002-9996-4429; Irle, Stephan/0000-0003-4995-4991 FU U.S. Department of Energy (DOE); Basic Energy Sciences (BES); Materials Sciences and Engineering Division; CREST (Core Research for Evolutional Science and Technology); Area of High Performance Computing for Multi-scale and Multiphysics Phenomena from the Japanese Science and Technology Agency (JST); Program for Improvement of Research Environment for Young Researchers from MEXT of Japan FX Experimental synthesis research supported by the U.S. Department of Energy (DOE), Basic Energy Sciences (BES), Materials Sciences and Engineering Division. Part of the computational calculations were conducted at the Center for Nanophase Materials Sciences (CNMS), and the electron microscopy characterization was performed at Oak Ridge National Laboratory's Shared Research Equipment (ShaRE) User Facility, both of which are sponsored by the Scientific User Facilities Division, DOE-BES. The theoretical work was in part supported by a CREST (Core Research for Evolutional Science and Technology) grant in the Area of High Performance Computing for Multi-scale and Multiphysics Phenomena from the Japanese Science and Technology Agency (JST). SI acknowledges support by the Program for Improvement of Research Environment for Young Researchers from MEXT of Japan. NR 52 TC 5 Z9 5 U1 2 U2 77 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2040-3364 EI 2040-3372 J9 NANOSCALE JI Nanoscale PY 2013 VL 5 IS 5 BP 1849 EP 1857 DI 10.1039/c2nr31788e PG 9 WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 089TC UT WOS:000314931900021 PM 23223914 ER PT J AU Yang, JB Zhai, DY Wang, HH Lau, KC Schlueter, JA Du, P Myers, DJ Sun, YK Curtiss, LA Amine, K AF Yang, Junbing Zhai, Dengyun Wang, Hsien-Hau Lau, Kah Chun Schlueter, John A. Du, Peng Myers, Deborah J. Sun, Yang-Kook Curtiss, Larry A. Amine, Khalil TI Evidence for lithium superoxide-like species in the discharge product of a Li-O-2 battery SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID AIR BATTERIES; ELECTRODES; STABILITY; DESIGN; OXIDES; CELLS AB We report on the use of a petroleum coke-based activated carbon (AC) with very high surface area for a Li-O-2 battery cathode without the use of any additional metal catalysts. Electrochemical measurement in a tetra(ethylene) glycol dimethyl ether-lithium triflate (TEGDME-LiCF3SO3) electrolyte results in two voltage plateaus during charging at 3.2-3.5 and 4.2-4.3 V versus Li+/Li. Herein we present evidence from Raman and magnetic measurements that the lower plateau corresponds to a form of lithium peroxide with superoxide-like properties characterized by a low temperature magnetic phase transition and a high O-O stretching frequency (1125 cm(-1)). The magnetic phase transition and the high O-O stretching frequency disappear when charged to above 3.7 V. Theoretical calculations indicate that a surface superoxide structure on lithium peroxide clusters and some lithium peroxide surfaces have an unpaired electron and a high O-O stretching frequency that help explain the observations. These results provide evidence that the form of the lithium peroxide discharge product is important to obtaining a low charge overpotential, and thus improving the round-trip efficiency between discharge and charge. C1 [Yang, Junbing; Zhai, Dengyun; Du, Peng; Myers, Deborah J.; Sun, Yang-Kook; Amine, Khalil] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Wang, Hsien-Hau; Lau, Kah Chun; Schlueter, John A.; Curtiss, Larry A.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Sun, Yang-Kook] Hanyang Univ, Dept Chem Engn, Seoul 133791, South Korea. [Curtiss, Larry A.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. RP Curtiss, LA (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM curtiss@anl.gov; amine@anl.gov RI Lau, Kah Chun/A-9348-2013; Du, Peng/F-8336-2013; Amine, Khalil/K-9344-2013 OI Lau, Kah Chun/0000-0002-4925-3397; FU U.S. Department of Energy Office of Basic Energy Science-Division of Materials Science [DE-AC02-06CH11357]; Human Resources Development of the Korea Institute of Energy Technology Evaluation of Planning (KETEP); Korea government of Ministry of Knowledge Economy [20114010203150] FX Support from the U.S. Department of Energy Office of Basic Energy Science-Division of Materials Science (grant number DE-AC02-06CH11357) is acknowledged. We acknowledge grants of computer time through the CNM Carbon Cluster at Argonne National Laboratory, the ALCF Fusion Cluster at Argonne National Laboratory. This work was also supported by the Human Resources Development of the Korea Institute of Energy Technology Evaluation of Planning (KETEP) grant funded by the Korea government of Ministry of Knowledge Economy (No. 20114010203150). The electron microscopy was accomplished at the Electron Microscopy Center for Materials Research at Argonne National Laboratory. NR 31 TC 100 Z9 100 U1 11 U2 196 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PY 2013 VL 15 IS 11 BP 3764 EP 3771 DI 10.1039/c3cp00069a PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 093AW UT WOS:000315165100009 PM 23389737 ER PT J AU Yee, SK Coates, NE Majumdar, A Urban, JJ Segalman, RA AF Yee, Shannon K. Coates, Nelson E. Majumdar, Arun Urban, Jeffrey J. Segalman, Rachel A. TI Thermoelectric power factor optimization in PEDOT:PSS tellurium nanowire hybrid composites SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID ELECTRICAL-CONDUCTIVITY; ENHANCEMENT; HETEROJUNCTIONS; NANOCOMPOSITES; THERMOPOWER; TRANSPORT; POLYMERS; FILMS AB The thermoelectric properties of a unique hybrid polymer-inorganic nanoparticle system consisting of tellurium nanowires and a conducting polymer, poly(3,4-ethylenedioxythiophene):poly(styrenesulfonate) (PEDOT:PSS), can be optimized by both controlling the shape of the nanoparticles and the loading and doping of the polymeric matrix with polar solvents. The mechanism for an observed improvement in power factor is attributed to the unique conducting nature of PEDOT:PSS, which exhibits a transition from a hopping transport-dominated regime to a carrier scattering-dominated regime upon doping with polar solvents. Near this transition, the electrical conductivity can be improved without significantly reducing the thermopower. Relying on this principle, the power factor optimization for this new thermoelectric material is experimentally carried out and found to exceed 100 mu W m(-1) K-2, which is nearly five orders of magnitude greater than pure PEDOT:PSS. C1 [Yee, Shannon K.; Majumdar, Arun] Univ Calif Berkeley, Dept Mech Engn, Berkeley, CA 94720 USA. [Yee, Shannon K.; Coates, Nelson E.; Urban, Jeffrey J.; Segalman, Rachel A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Coates, Nelson E.; Segalman, Rachel A.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. RP Urban, JJ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, 1 Cyclotron Rd,Mail Stop 67R4110, Berkeley, CA 94720 USA. EM shannon.yee@berkeley.edu; necoates@lbl.gov; 4majumdar.pubs@gmail.com; jjurban@lbl.gov; segalman@berkeley.edu RI Foundry, Molecular/G-9968-2014; OI Segalman, Rachel/0000-0002-4292-5103 FU Department of Energy BES-LBL Thermoelectrics Program [DE-AC02-05CH11231]; Office of Science, Office of Basic Energy Sciences, Scientific User Facilities Division, of the U.S. Department of Energy [DE-AC02-05CH11231]; John and Fannie Hertz Foundation; Big George Fellowship FX We gratefully acknowledge support through the Department of Energy BES-LBL Thermoelectrics Program under Contract No. DE-AC02-05CH11231. This work was partially performed at the Molecular Foundry, Lawrence Berkeley National Laboratory, and was supported by the Office of Science, Office of Basic Energy Sciences, Scientific User Facilities Division, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. We also thank Prof. Chris Dames, Boris Russ, and Adrianne Rosales for their insight and conversations during the execution of this work. S. K. Yee acknowledges support from the John and Fannie Hertz Foundation and the Big George Fellowship. NR 40 TC 53 Z9 53 U1 7 U2 163 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PY 2013 VL 15 IS 11 BP 4024 EP 4032 DI 10.1039/c3cp44558e PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 093AW UT WOS:000315165100037 PM 23400218 ER PT J AU Goulay, F Derakhshan, A Maher, E Trevitt, AJ Savee, JD Scheer, AM Osborn, DL Taatjes, CA AF Goulay, Fabien Derakhshan, Adeeb Maher, Eamonn Trevitt, Adam J. Savee, John D. Scheer, Adam M. Osborn, David L. Taatjes, Craig A. TI Formation of dimethylketene and methacrolein by reaction of the CH radical with acetone SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID CROSS-SECTIONS; RATE-CONSTANT; 248 NM; PHOTOIONIZATION; KINETICS; ACETALDEHYDE; ALDEHYDES; PROPYNE; SERIES; KETENE AB The reaction of the methylidyne radical (CH) with acetone ((CH3)(2)C=O) is studied at room temperature and at a pressure of 4 Torr (533.3 Pa) using a multiplexed photoionization mass spectrometer coupled to the tunable vacuum ultraviolet synchrotron radiation of the Advanced Light Source at Lawrence Berkeley National Laboratory. The CH radicals are generated by 248 nm multiphoton photolysis of bromoform and react with acetone in an excess of helium and nitrogen gas flow. The main observed reaction exit channel is elimination of a hydrogen atom to form C4H6O isomers. Analysis of photoionization spectra identifies dimethylketene and methacrolein as the only H-elimination products. The best fit to the data gives branching ratios of 0.68 +/- 0.14 for methacrolein and 0.32 +/- 0.07 for dimethylketene. A methylketene spectrum measured here is used to reanalyze the photoionization spectrum obtained at m/z = 56 for the CH + acetaldehyde reaction, (Goulay et al., J. Phys. Chem. A, 2012, 116, 6091) yielding new H-loss branching ratios of 0.61 +/- 0.12 for acrolein and 0.39 +/- 0.08 for methylketene. The contribution from methyleneoxirane to the reaction product distribution is revised to be negligible. Coupled with additional product detection for the CD + acetone reaction, these observations pave the way for development of general set of reaction mechanisms for the addition of CH to compounds containing an acetyl subgroup. C1 [Goulay, Fabien; Derakhshan, Adeeb; Maher, Eamonn] W Virginia Univ, Dept Chem, Morgantown, WV 26506 USA. [Trevitt, Adam J.] Univ Wollongong, Sch Chem, Wollongong, NSW 2522, Australia. [Savee, John D.; Scheer, Adam M.; Osborn, David L.; Taatjes, Craig A.] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA. RP Goulay, F (reprint author), W Virginia Univ, Dept Chem, Morgantown, WV 26506 USA. EM Fabien.goulay@mail.wvu.edu RI Trevitt, Adam/A-2915-2009; OI Trevitt, Adam/0000-0003-2525-3162; Derakhshan, Adeeb/0000-0003-4324-8113 FU West Virginia University; Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy at Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; Australian Research Council [DP1094135]; International Synchrotron Access Program (ISAP); Federal Government of Australia; Division of Chemical Sciences, Geosciences, and Biosciences, the Office of Basic Energy Sciences, the U. S. Department of Energy; National Nuclear Security Administration [DE-AC04-94-AL85000] FX F.G., A. D. and E. M. acknowledge West Virginia University for funding (start up package, F. G.). The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231 at Lawrence Berkeley National Laboratory. A.J.T. acknowledges funding support from the Australian Research Council (DP1094135) and travel funding provided by the International Synchrotron Access Program (ISAP) managed by the Australian Synchrotron. The ISAP is funded by a National Collaborative Research Infrastructure Strategy grant provided by the Federal Government of Australia. We thank Mr Howard Johnsen for technical support of this experiment. We also thank Dr Doug Taube for his help during the ketene synthesis. Sandia authors (J.D.S., A. M. S, D.L.O., C. A. T.) and the instrumentation for this work are supported by the Division of Chemical Sciences, Geosciences, and Biosciences, the Office of Basic Energy Sciences, the U. S. Department of Energy. Sandia is a multi-program laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the National Nuclear Security Administration under contract DE-AC04-94-AL85000. We thank Dr Oliver Welz for the experimental absolute photoionization spectrum of methacrolein. NR 46 TC 9 Z9 9 U1 5 U2 60 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PY 2013 VL 15 IS 11 BP 4049 EP 4058 DI 10.1039/c3cp43829e PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 093AW UT WOS:000315165100040 PM 23403615 ER PT J AU Yang, SY Yu, HD Chen, YX He, F Li, X Lu, K AF Yang, Shangyuan Yu, Huadong Chen, Yingxu He, Feng Li, Xin Lu, Kang TI The degradation pathway of aminosilicone polymer in aqueous microemulsion by Fenton process SO POLYMER DEGRADATION AND STABILITY LA English DT Article DE Aminosilicone polymers (PDMAS); Degradation pathway; Fenton reaction; Oxidation; Coagulation ID HYDROXYL RADICALS; WASTE-WATER; NONIONIC SURFACTANTS; OXIDATION; KINETICS; OZONE; POLYDIMETHYLSILOXANES; REACTIVITY; SILICONES; REMOVAL AB This research systematically studied the degradation pathway of aminosilicone polymers (PDMAS) by Fenton process in aqueous microemulsion. We show that the optimum parameters of Fenton process for degradation of PDMAS and COD reduction in aqueous microemulsion (COD = 4500 mg/L) are pH of 2.5, ferrous iron of 5 mM, and hydrogen peroxide of 10 mM. Under optimal reaction conditions and with pH modified to 8 after Fenton reactions, 42 mg/L NH4+ was produced along with 76.8% COD removal, in which oxidation and coagulation contributed 10.6% and 66.2%, respectively. Yet, COD removal of PDMAS emulsion by same amount of ferric ions at pH 8 was only 5.7%, indicating the major removal of COD was through precipitation of PDMAS and its oxidation intermediates from Fenton reaction due to the destabilization of the microelumsion resulted from surfactant degradation. Comparison of the FTIR spectra before and after treatment by Fenton process revealed the absence of amine groups on side chains, which suggested the complete break down of the C-N bonds by hydroxyl radicals. GPC results further showed that the backbone of PDMAS was likely broken down randomly, resulting in intermediates with lower molecular weights. (C) 2012 Published by Elsevier Ltd. C1 [Yang, Shangyuan; Yu, Huadong; Chen, Yingxu; Li, Xin; Lu, Kang] Zhejiang Univ, Dept Environm Engn, Key Lab Water Polluting Control & Environm Safety, Hangzhou, Zhejiang, Peoples R China. [He, Feng] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. RP Chen, YX (reprint author), Zhejiang Univ, Dept Environm Engn, Key Lab Water Polluting Control & Environm Safety, Hangzhou, Zhejiang, Peoples R China. EM yingxuchen@zju.edu.cn; hef2@oml.gov FU Key Science and Technology Project of Zhejiang Province [2010C13002] FX This research was funded by the Key Science and Technology Project of Zhejiang Province (2010C13002). We would also like to thank Transfar Group Corporation for providing the PDMAS samples and other assistances for this research. NR 34 TC 1 Z9 1 U1 4 U2 34 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0141-3910 J9 POLYM DEGRAD STABIL JI Polym. Degrad. Stabil. PD JAN PY 2013 VL 98 IS 1 BP 464 EP 470 DI 10.1016/j.polymdegradstab.2012.06.032 PG 7 WC Polymer Science SC Polymer Science GA 093DD UT WOS:000315171000056 ER PT J AU Green, MA Emery, K Hishikawa, Y Warta, W Dunlop, ED AF Green, Martin A. Emery, Keith Hishikawa, Yoshihiro Warta, Wilhelm Dunlop, Ewan D. TI Solar cell efficiency tables (version 41) SO PROGRESS IN PHOTOVOLTAICS LA English DT Article DE solar cell efficiency; photovoltaic efficiency; energy conversion efficiency ID MULTICRYSTALLINE; CONCENTRATOR; STABILITY AB Consolidated tables showing an extensive listing of the highest independently confirmed efficiencies for solar cells and modules are presented. Guidelines for inclusion of results into these tables are outlined, and new entries since June 2012 are reviewed. Copyright (C) 2012 John Wiley & Sons, Ltd. C1 [Green, Martin A.] Univ New S Wales, Australian Ctr Adv Photovolta, Sydney, NSW 2052, Australia. [Emery, Keith] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Hishikawa, Yoshihiro] Natl Inst Adv Ind Sci & Technol, Res Ctr Photovolta RCPV, Tsukuba, Ibaraki 3058568, Japan. [Warta, Wilhelm] Fraunhofer Inst Solar Energy Syst, Dept Solar Cells Mat & Technol, D-79110 Freiburg, Germany. [Dunlop, Ewan D.] Commiss European Communities, Joint Res Ctr, Renewable Energy Unit, Inst Energy, IT-21027 Ispra, VA, Italy. RP Green, MA (reprint author), Univ New S Wales, ARC Photovolta Ctr Excellence, Sydney, NSW 2052, Australia. EM m.green@unsw.edu.au FU Australian Solar Institute FX The Australian Centre for Advanced Photovoltaics commenced in January 2013 with support from the Australian Solar Institute. NR 46 TC 432 Z9 440 U1 12 U2 443 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1062-7995 J9 PROG PHOTOVOLTAICS JI Prog. Photovoltaics PD JAN PY 2013 VL 21 IS 1 BP 1 EP 11 DI 10.1002/pip.2352 PG 11 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA 095IP UT WOS:000315328200001 ER PT J AU Jordan, DC Kurtz, SR AF Jordan, D. C. Kurtz, S. R. TI Photovoltaic Degradation Rates-an Analytical Review SO PROGRESS IN PHOTOVOLTAICS LA English DT Review DE photovoltaic modules; photovoltaic systems; performance; outdoor testing; field testing; degradation rates ID CONNECTED PV SYSTEMS; AMORPHOUS-SILICON; PERFORMANCE ANALYSIS; OUTDOOR PERFORMANCE; SOLAR-ENERGY; LARGE-SCALE; MODULES; RELIABILITY; EXPERIENCE; EXPOSURE AB As photovoltaic penetration of the power grid increases, accurate predictions of return on investment require accurate prediction of decreased power output over time. Degradation rates must be known in order to predict power delivery. This article reviews degradation rates of flat-plate terrestrial modules and systems reported in published literature from field testing throughout the last 40 years. Nearly 2000 degradation rates, measured on individual modules or entire systems, have been assembled from the literature, showing a median value of 0.5%/year. The review consists of three parts: a brief historical outline, an analytical summary of degradation rates, and a detailed bibliography partitioned by technology. Copyright (C) 2011 John Wiley & Sons, Ltd. C1 [Jordan, D. C.; Kurtz, S. R.] Natl Renewable Energy Lab NREL, Golden, CO 80401 USA. RP Jordan, DC (reprint author), Natl Renewable Energy Lab NREL, Natl Ctr Photovolta, 1617 Cole Blvd, Golden, CO 80401 USA. EM dirk.jordan@nrel.gov FU U.S. Department of Energy [DE-AC36-08-GO28308]; National Renewable Energy Laboratory FX We would like to thank John Wohlgemuth for the review of the manuscript and the rest of NREL's Reliability group for helpful discussions. This work was supported by the U.S. Department of Energy under contract no. DE-AC36-08-GO28308 with the National Renewable Energy Laboratory. NR 168 TC 149 Z9 150 U1 11 U2 88 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1062-7995 EI 1099-159X J9 PROG PHOTOVOLTAICS JI Prog. Photovoltaics PD JAN PY 2013 VL 21 IS 1 BP 12 EP 29 DI 10.1002/pip.1182 PG 18 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA 095IP UT WOS:000315328200002 ER PT J AU Dyer, C Jiang, Z Bozell, J Rials, T Heller, WT Dadmun, M AF Dyer, Caleb Jiang, Zhe Bozell, Joe Rials, Timothy Heller, William T. Dadmun, Mark TI Effect of chain structure on the miscibility of cellulose acetate blends: a small-angle neutron scattering study SO SOFT MATTER LA English DT Article ID POLY(2,6-DIMETHYL-1,4-PHENYLENE OXIDE); PHASE-SEPARATION; CO-POLYMERS; BIODEGRADATION; POLYSTYRENE; PROPIONATE; COPOLYMERS; BEHAVIOR; THERMODYNAMICS; SPECTROSCOPY AB The miscibility of cellulose ester blends with varying degree of substitution (DS) of acetates along the chain backbone has been investigated using small-angle neutron scattering. The difference in degree of substitution (Delta DS) between the two components in the blend was systematically varied from 0.06 to 0.63 where each blend was found to be a partially miscible, two-phase system. Miscibility between the two components initially decreases as Delta DS of the blends increases. The Flory interaction parameter, c, concurrently increases with increasing Delta DS as a result of diminishing van der Waals forces between components. The cellulose acetates with lower degree of substitution, which contain more hydroxyl substituents, however, demonstrate greater miscibility even at higher Delta DS. This is interpreted to be the result of favorable hydrogen bonding between blend components that are possible in the presence of more hydroxyl groups. FT-IR data support this interpretation, indicating an increase in hydrogen bonding in a blend having a lower DS component. These results indicate that while an increase in structural differences between cellulose acetate blend components limits miscibility, the presence of hydroxyl groups on the chain promotes mixing. This competition accentuates the significant impact specific interactions have on blend miscibility for these copolymers. C1 [Dyer, Caleb; Dadmun, Mark] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Dadmun, Mark] Oak Ridge Natl Lab, Chem Sci Div, Oak Ridge, TN 37831 USA. [Jiang, Zhe; Bozell, Joe; Rials, Timothy] Univ Tennessee, Biomass Chem Labs, Ctr Renewable Carbon, Knoxville, TN 37996 USA. [Heller, William T.] Univ Tennessee, Ctr Struct Mol Biol, Knoxville, TN 37996 USA. [Heller, William T.] Univ Tennessee, Biol & Soft Matter Div, Knoxville, TN 37996 USA. RP Dadmun, M (reprint author), Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. EM Dad@utk.edu FU Department of Energy, Office of Basic Sciences, through the EPSCoR [DE-FG02-08ER46528]; Joint Institute for Neutron Sciences at the University of Tennessee; U.S. Department of Energy's Office of Biological and Environmental Research [FWP ERKP291]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX This work was supported by the Department of Energy, Office of Basic Sciences, through the EPSCoR grant, DE-FG02-08ER46528. The authors also wish to acknowledge the Joint Institute for Neutron Sciences at the University of Tennessee for support of this project. The research at ORNL's Center for Structural Molecular Biology (FWP ERKP291) was supported by the U.S. Department of Energy's Office of Biological and Environmental Research. A portion of this research at Oak Ridge National Laboratory's High Flux Isotope Reactor was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. NR 34 TC 2 Z9 2 U1 1 U2 16 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1744-683X J9 SOFT MATTER JI Soft Matter PY 2013 VL 9 IS 12 BP 3402 EP 3411 DI 10.1039/c3sm27648a PG 10 WC Chemistry, Physical; Materials Science, Multidisciplinary; Physics, Multidisciplinary; Polymer Science SC Chemistry; Materials Science; Physics; Polymer Science GA 096NR UT WOS:000315411700021 ER PT J AU Khangaonkar, T Wang, TP AF Khangaonkar, Tarang Wang, Taiping TI Potential alteration of fjordal circulation due to a large floating structure-Numerical investigation with application to Hood Canal basin in Puget Sound SO APPLIED OCEAN RESEARCH LA English DT Article DE 3D hydrodynamic model; Unstructured grid; FVCOM; Fjords; Partially mixed estuaries; Analytical solution; Estuarine circulation; Hood Canal; Puget; Sound; Salish Sea ID COASTAL OCEAN MODEL; FINITE-VOLUME; RESIDUAL CIRCULATION; SHALLOW ESTUARIES; NARROW ESTUARIES; BAY; ZONES AB Circulation in typical fjords is characterized by a shallow brackish layer at the surface over a deep long and narrow saltwater column. This surface layer is responsible for the outflow of water from the fjord and is important for flushing of the basin and water quality maintenance. The vertical structure of circulation and transport is known to be easily disrupted, and we postulate that the stability of fjordal circulation may also be vulnerable to impacts from anthropogenic alterations, such as floating structures, which could constrict the mixing and transport in the upper layers of the water column. First, using simplified fjord geometry and a three-dimensional finite volume coastal ocean model (FVCOM), a baseline examination of tidally averaged current profiles in basins with and without sills is presented. The response, varying from a partially mixed estuary regime to classical fjord conditions matches many fjord-like basins such as those in Puget Sound, Washington. The effect of surface obstruction on tidally averaged currents and residence times was then examined by incorporation of a narrow block in the surface layer of the model across the width of the simplified fjord channel such that normal velocity in the horizontal direction was forced to zero. This block approximated the presence of a floating bridge and was further tested using the geometry of Hood Canal, a fjordal sub-basin with a sill in Puget Sound. The results show that tidally averaged mean outflow under the influence of such a constraint at the water surface could be reduced significantly. In the case of Hood Canal, preliminary results indicate that the presence of the floating bridge might have increased the residence times in the basin by 8-13%, which could be an important factor affecting water quality. (C) 2012 Elsevier Ltd. All rights reserved. C1 [Khangaonkar, Tarang; Wang, Taiping] Pacific NW Natl Lab, Marine Sci Div, Seattle, WA 98109 USA. RP Khangaonkar, T (reprint author), Pacific NW Natl Lab, Marine Sci Div, 1100 Dexter Ave N,Suite 400, Seattle, WA 98109 USA. EM tarang.khangaonkar@pnnl.gov FU Washington State Department of Ecology; U.S. Environmental Protection Agency FX This work would not have been possible without technical input and advice from our colleagues Dr. Wen Long and Dr. Taeyun Kim. Similarly we would like to thank our senior scientists Dr. Charlie Brandt and Dr. Gary Gill for reviewing the document and providing many helpful comments. We would also like to acknowledge our collaborators from the Washington State Department of Ecology and from the U.S. Environmental Protection Agency for their encouragement and support. NR 47 TC 0 Z9 0 U1 1 U2 11 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0141-1187 J9 APPL OCEAN RES JI Appl. Ocean Res. PD JAN PY 2013 VL 39 BP 146 EP 157 DI 10.1016/j.apor.2012.11.003 PG 12 WC Engineering, Ocean; Oceanography SC Engineering; Oceanography GA 091VG UT WOS:000315077300016 ER PT J AU Melton, JR Wania, R Hodson, EL Poulter, B Ringeval, B Spahni, R Bohn, T Avis, CA Beerling, DJ Chen, G Eliseev, AV Denisov, SN Hopcroft, PO Lettenmaier, DP Riley, WJ Singarayer, JS Subin, ZM Tian, H Zurcher, S Brovkin, V van Bodegom, PM Kleinen, T Yu, ZC Kaplan, JO AF Melton, J. R. Wania, R. Hodson, E. L. Poulter, B. Ringeval, B. Spahni, R. Bohn, T. Avis, C. A. Beerling, D. J. Chen, G. Eliseev, A. V. Denisov, S. N. Hopcroft, P. O. Lettenmaier, D. P. Riley, W. J. Singarayer, J. S. Subin, Z. M. Tian, H. Zuercher, S. Brovkin, V. van Bodegom, P. M. Kleinen, T. Yu, Z. C. Kaplan, J. O. TI Present state of global wetland extent and wetland methane modelling: conclusions from a model inter-comparison project (WETCHIMP) SO BIOGEOSCIENCES LA English DT Article ID ATMOSPHERIC METHANE; NATURAL WETLANDS; ELEVATED CO2; NORTHERN WETLANDS; CH4 EMISSIONS; BIOGEOCHEMISTRY MODEL; CLIMATE FEEDBACKS; ISOTOPE STAGE-3; RICE PADDIES; CARBON-CYCLE AB Global wetlands are believed to be climate sensitive, and are the largest natural emitters of methane (CH4). Increased wetland CH4 emissions could act as a positive feedback to future warming. The Wetland and Wetland CH4 Inter-comparison of Models Project (WETCHIMP) investigated our present ability to simulate large-scale wetland characteristics and corresponding CH4 emissions. To ensure inter-comparability, we used a common experimental protocol driving all models with the same climate and carbon dioxide (CO2) forcing datasets. The WETCHIMP experiments were conducted for model equilibrium states as well as transient simulations covering the last century. Sensitivity experiments investigated model response to changes in selected forcing inputs (precipitation, temperature, and atmospheric CO2 concentration). Ten models participated, covering the spectrum from simple to relatively complex, including models tailored either for regional or global simulations. The models also varied in methods to calculate wetland size and location, with some models simulating wetland area prognostically, while other models relied on remotely sensed inundation datasets, or an approach intermediate between the two. Four major conclusions emerged from the project. First, the suite of models demonstrate extensive disagreement in their simulations of wetland areal extent and CH4 emissions, in both space and time. Simple metrics of wetland area, such as the latitudinal gradient, show large variability, principally between models that use inundation dataset information and those that independently determine wetland area. Agreement between the models improves for zonally summed CH4 emissions, but large variation between the models remains. For annual global CH4 emissions, the models vary by +/- 40% of the all-model mean (190 Tg CH4 yr(-1)). Second, all models show a strong positive response to increased atmospheric CO2 concentrations (857 ppm) in both CH4 emissions and wetland area. In response to increasing global temperatures (+3.4 degrees C globally spatially uniform), on average, the models decreased wetland area and CH4 fluxes, primarily in the tropics, but the magnitude and sign of the response varied greatly. Models were least sensitive to increased global precipitation (+3.9% globally spatially uniform) with a consistent small positive response in CH4 fluxes and wetland area. Results from the 20th century transient simulation show that interactions between climate forcings could have strong non-linear effects. Third, we presently do not have sufficient wetland methane observation datasets adequate to evaluate model fluxes at a spatial scale comparable to model grid cells (commonly 0.5 degrees). This limitation severely restricts our ability to model global wetland CH4 emissions with confidence. Our simulated wetland extents are also difficult to evaluate due to extensive disagreements between wetland mapping and remotely sensed inundation datasets. Fourth, the large range in predicted CH4 emission rates leads to the conclusion that there is both substantial parameter and structural uncertainty in large-scale CH4 emission models, even after uncertainties in wetland areas are accounted for. C1 [Melton, J. R.; Kaplan, J. O.] Ecole Polytech Fed Lausanne, ARVE Grp, CH-1015 Lausanne, Switzerland. [Wania, R.] Univ Montpellier 2, CNRS, UMR 5554, Inst Sci Evolut, F-34090 Montpellier, France. [Poulter, B.; Ringeval, B.] UVSQ, CNRS, CEA, Lab Sci Climat & Environm, Gif Sur Yvette, France. [Ringeval, B.; Hopcroft, P. O.; Singarayer, J. S.] Univ Bristol, Sch Geog Sci, BRIDGE, Bristol BS8 1TH, Avon, England. [Ringeval, B.] Vrije Univ Amsterdam, Dept Earth Sci, Amsterdam, Netherlands. [Spahni, R.; Zuercher, S.] Univ Bern, Inst Phys, CH-3012 Bern, Switzerland. [Spahni, R.; Zuercher, S.] Univ Bern, Oeschger Ctr Climate Change Res, CH-3012 Bern, Switzerland. [Bohn, T.; Lettenmaier, D. P.] Univ Washington, Dept Civil & Environm Engn, Seattle, WA 98195 USA. [Avis, C. A.] Univ Victoria, Sch Earth & Ocean Sci, Victoria, BC V8W 2Y2, Canada. [Beerling, D. J.] Univ Sheffield, Dept Anim & Plant Sci, Sheffield S10 2TN, S Yorkshire, England. [Chen, G.; Tian, H.] Auburn Univ, Int Ctr Climate & Global Change Res, Auburn, AL 36849 USA. [Eliseev, A. V.; Denisov, S. N.] Russian Acad Sci, AM Obukhov Inst Atmospher Phys, Moscow 117901, Russia. [Eliseev, A. V.] Kazan Volga Reg Fed Univ, Kazan, Russia. [Riley, W. J.; Subin, Z. M.] Lawrence Berkeley Natl Lab, ESD, Berkeley, CA USA. [Brovkin, V.; Kleinen, T.] Max Planck Inst Meteorol, D-20146 Hamburg, Germany. [van Bodegom, P. M.] Vrije Univ Amsterdam, Dept Ecol Sci, Amsterdam, Netherlands. [Yu, Z. C.] Lehigh Univ, Dept Earth & Environm Sci, Bethlehem, PA USA. RP Melton, JR (reprint author), Environm Canada, Canadian Ctr Climate Modelling & Anal, Victoria, BC V8W 2Y2, Canada. EM joe.melton.sci@gmail.com RI Riley, William/D-3345-2015; Yu, Zicheng/D-4108-2012; Brovkin, Victor/C-2803-2016; Kaplan, Jed/P-1796-2015; Hopcroft, Peter/H-4957-2016; Eliseev, Alexey V./L-8707-2013; Tian, Hanqin/A-6484-2012; lettenmaier, dennis/F-8780-2011; Denisov, Sergey/N-2700-2013; Brovkin, Victor/I-7450-2012; Subin, Zachary/K-5168-2012; Bohn, Theodore/K-4494-2012; van Bodegom, Peter/N-8150-2015 OI Ringeval, Bruno/0000-0001-8405-1304; Riley, William/0000-0002-4615-2304; Brovkin, Victor/0000-0001-6420-3198; Kaplan, Jed/0000-0001-9919-7613; Hopcroft, Peter/0000-0003-3694-9181; Eliseev, Alexey V./0000-0001-7288-7649; Tian, Hanqin/0000-0002-1806-4091; lettenmaier, dennis/0000-0003-3317-1327; Subin, Zachary/0000-0002-9257-9288; Bohn, Theodore/0000-0002-1880-9129; van Bodegom, Peter/0000-0003-0771-4500 FU COST Action [ES0805]; Swiss Ministry for Research and Education [C09.0054]; Swiss National Science Foundation [PP0022_119049, PP00P2_39193]; Office of Science, Office of Biological and Environmental Research, Climate and Environmental Science Division, of the US Department of Energy [DE-AC02-05CH11231]; NASA's ROSES program [NNX08AH97G]; US NSF [ARC-1107981]; The Max Planck Society (Germany); President of Russia grant [5467.2012.5]; Russian Foundation for Basic Research; Russian Academy of Sciences; Swiss National Science Foundation; European Research Council (ERC) under European Community [226172]; NERC UK [NE/I010912/1]; NERC UK/INSU France QUEST-DESIRE project; ETH Competence Center Environment and Sustainability FX The authors are grateful to the COST Action ES0805 TERRABITES for providing support for the WETCHIMP workshop. We thank Sylvia Houston and Olga Petrikova for assistance with organizing the project meeting and Kristen Krumhardt for assistance producing the figures. J. R. M. was supported by the Swiss Ministry for Research and Education (grant C09.0054). J. O. K. acknowledges support from the Swiss National Science Foundation (grant PP0022_119049 and PP00P2_39193). The contributions of W. J. R. and Z. M. S. were supported by the Director, Office of Science, Office of Biological and Environmental Research, Climate and Environmental Science Division, of the US Department of Energy under Contract No. DE-AC02-05CH11231 to Berkeley Lab (IMPACTS and C-Climate Uncertainties projects). The contributions of T. J. B. and D. P. L. were supported by NASA's ROSES program, grant NNX08AH97G. The contribution of Z. C. Y. was supported by a US NSF grant (ARC-1107981) and a grant from The Max Planck Society (Germany). A. V. E. and S. N. D. were supported by the the President of Russia grant 5467.2012.5, by the Russian Foundation for Basic Research, and by the programs of the Russian Academy of Sciences. The contributions of R. S. and S. Z. were supported by the Swiss National Science Foundation and by the European Research Council advanced grant MATRICs (ERC grant agreement no. 226172) under the European Community's Seventh Framework Programme. P. O. H. is supported by a NERC UK grant NE/I010912/1 and previously through NERC UK/INSU France QUEST-DESIRE project. E. L. H. was supported by ETH Competence Center Environment and Sustainability's grant MAIOLICA. H. T. and G. C. wish to thank Xiaofeng Xu for assistance with formatting inputs and setting up earlier DLEM model simulations. We thank two anonymous referees for their comments that improved this manuscript. NR 140 TC 122 Z9 125 U1 21 U2 173 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1726-4170 EI 1726-4189 J9 BIOGEOSCIENCES JI Biogeosciences PY 2013 VL 10 IS 2 BP 753 EP 788 DI 10.5194/bg-10-753-2013 PG 36 WC Ecology; Geosciences, Multidisciplinary SC Environmental Sciences & Ecology; Geology GA 092BE UT WOS:000315093000008 ER PT J AU Mu, QZ Zhao, MS Kimball, JS McDowell, NG Running, SW AF Mu, Qiaozhen Zhao, Maosheng Kimball, John S. McDowell, Nathan G. Running, Steven W. TI A REMOTELY SENSED GLOBAL TERRESTRIAL DROUGHT SEVERITY INDEX SO BULLETIN OF THE AMERICAN METEOROLOGICAL SOCIETY LA English DT Article ID NET PRIMARY PRODUCTION; EVAPOTRANSPIRATION ALGORITHM; SURFACE-TEMPERATURE; INDUCED REDUCTION; VEGETATION INDEX; FLUX MEASUREMENT; SOIL-MOISTURE; UNITED-STATES; HEAT-FLUX; DATA SET C1 [Mu, Qiaozhen; Zhao, Maosheng; Running, Steven W.] Univ Montana, Numer Terradynam Simulat Grp, Coll Forestry & Conservat, Missoula, MT 59812 USA. [Kimball, John S.] Univ Montana, Flathead Lake Biol Stn, Polson, MT 59860 USA. [McDowell, Nathan G.] Los Alamos Natl Lab, Atmospher & Environm Dynam Grp, Los Alamos, NM USA. RP Mu, QZ (reprint author), Univ Montana, Numer Terradynam Simulat Grp, Coll Forestry & Conservat, 32 Campus Dr, Missoula, MT 59812 USA. EM qiaozhen@ntsg.umt.edu RI Zhao, Maosheng/G-5706-2010; Mu, Qiaozhen/G-5695-2010 FU NASA Earth Observing System MODIS project [NNH09ZDA001N-TERRA-AQUA] FX This work is funded by the NASA Earth Observing System MODIS project (Grant NNH09ZDA001N-TERRA-AQUA). We thank the anonymous reviewers, as well as communications with Dr. Michael J. Hayes at the University of Nebraska at Lincoln. The shapefile for Amazon is provided by Dr. Simon L. Lewis. NR 98 TC 82 Z9 88 U1 10 U2 76 PU AMER METEOROLOGICAL SOC PI BOSTON PA 45 BEACON ST, BOSTON, MA 02108-3693 USA SN 0003-0007 J9 B AM METEOROL SOC JI Bull. Amer. Meteorol. Soc. PD JAN PY 2013 VL 94 IS 1 BP 83 EP 98 DI 10.1175/BAMS-D-11-00213.1 PG 16 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 087QG UT WOS:000314776500009 ER PT J AU Kim, SK Hay, BP Kim, JS Moyer, BA Sessler, JL AF Kim, Sung Kuk Hay, Benjamin P. Kim, Jong Seung Moyer, Bruce A. Sessler, Jonathan L. TI Capture and metathesis-based release of potassium salts by a multitopic ion receptor SO CHEMICAL COMMUNICATIONS LA English DT Article ID ALKALI-METAL CATIONS; PAIR RECEPTOR; CATION/ETHER COMPLEXES; MOLECULAR RECOGNITION; BINDING; TRANSPORT; MEMBRANE; CHANNELS; DOUBLE-1,3-ALTERNATE-CALIXCROWN; MULTI-1,3-ALTERNATE-CALIXCROWN AB The multitopic ion-pair receptor 2 is able to recognize and extract various cesium and potassium salts via three different ion recognition modes. Furthermore, it is capable of extracting and then releasing KNO3 via ion-pair metathesis with CsClO4, allowing KNO3 recovery. C1 [Kim, Sung Kuk; Sessler, Jonathan L.] Univ Texas Austin, Dept Chem & Biochem, Austin, TX 78712 USA. [Hay, Benjamin P.; Moyer, Bruce A.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37830 USA. [Kim, Jong Seung] Korea Univ, Dept Chem, Seoul 136701, South Korea. [Sessler, Jonathan L.] Yonsei Univ, Dept Chem, Seoul 120749, South Korea. RP Hay, BP (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37830 USA. EM sessler@cm.utexas.edu RI Kim, Jong Seung/N-4504-2015; Moyer, Bruce/L-2744-2016 OI Kim, Jong Seung/0000-0003-3477-1172; Moyer, Bruce/0000-0001-7484-6277 FU Office of Basic Energy Sciences, U.S. Department of Energy (DOE) [DE-FG02-01ER15186]; CRI project of KRF [20120000243]; Korean WCU program [R32-2010-000-10217-0]; Ministry of Education, Science and Technology (MEST); Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. DOE FX This work was supported by the Office of Basic Energy Sciences, U.S. Department of Energy (DOE) (grant DE-FG02-01ER15186 to J.L.S.), CRI project of KRF (No. 20120000243 to J.S.K), and the Korean WCU program (R32-2010-000-10217-0) administered through the National Research Foundation of Korea funded by the Ministry of Education, Science and Technology (MEST). B.P.H. and B.A.M. acknowledge support from the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. DOE. NR 37 TC 9 Z9 9 U1 1 U2 40 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1359-7345 J9 CHEM COMMUN JI Chem. Commun. PY 2013 VL 49 IS 21 BP 2112 EP 2114 DI 10.1039/c3cc39117e PG 3 WC Chemistry, Multidisciplinary SC Chemistry GA 089ER UT WOS:000314893200005 PM 23389421 ER PT J AU Chorin, AJ Morzfeld, M Tu, XM AF Chorin, Alexandre J. Morzfeld, Matthias Tu, Xuemin TI Implicit Sampling, with Application to Data Assimilation SO CHINESE ANNALS OF MATHEMATICS SERIES B LA English DT Article DE Importance sampling; Bayesian estimation; Particle filter; Implicit filter; Data assimilation ID VARIATIONAL ASSIMILATION; PARTICLE FILTERS; IMPLEMENTATION; EQUATIONS; SYSTEMS; 4D-VAR; NOISE; MODEL AB There are many computational tasks, in which it is necessary to sample a given probability density function (or pdf for short), i.e., to use a computer to construct a sequence of independent random vectors x (i) (i = 1, 2, aEuro broken vertical bar), whose histogram converges to the given pdf. This can be difficult because the sample space can be huge, and more importantly, because the portion of the space, where the density is significant, can be very small, so that one may miss it by an ill-designed sampling scheme. Indeed, Markovchain Monte Carlo, the most widely used sampling scheme, can be thought of as a search algorithm, where one starts at an arbitrary point and one advances step-by-step towards the high probability region of the space. This can be expensive, in particular because one is typically interested in independent samples, while the chain has a memory. The authors present an alternative, in which samples are found by solving an algebraic equation with a random right-hand side rather than by following a chain; each sample is independent of the previous samples. The construction in the context of numerical integration is explained, and then it is applied to data assimilation. C1 [Chorin, Alexandre J.] Univ Calif Berkeley, Dept Math, Berkeley, CA 94720 USA. [Chorin, Alexandre J.; Morzfeld, Matthias] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Tu, Xuemin] Univ Kansas, Dept Math, Lawrence, KS 66045 USA. RP Chorin, AJ (reprint author), Univ Calif Berkeley, Dept Math, Berkeley, CA 94720 USA. EM chorin@math.berkeley.edu; mmo@math.lbl.gov; xtu@math.ku.edu FU National Science Foundation [DMS-0705910, OCE-0934298]; Office of Science, Computational and Technology Research, U.S. Department of Energy [DE-AC02-05CH11231] FX Project supported by the Director, Office of Science, Computational and Technology Research, U.S. Department of Energy (No. DE-AC02-05CH11231) and the National Science Foundation (Nos. DMS-0705910, OCE-0934298). NR 34 TC 1 Z9 1 U1 2 U2 5 PU SHANGHAI SCIENTIFIC TECHNOLOGY LITERATURE PUBLISHING HOUSE PI SHANGHAI PA SHANGHAI, PEOPLES R CHINA SN 0252-9599 EI 1860-6261 J9 CHINESE ANN MATH B JI Chin. Ann. Math. Ser. B PD JAN PY 2013 VL 34 IS 1 BP 89 EP 98 DI 10.1007/s11401-012-0757-5 PG 10 WC Mathematics SC Mathematics GA 079QY UT WOS:000314188000004 ER PT J AU Ning, FL Zhang, KN Wu, NY Jiang, GS Zhang, L Liu, L Yu, YB AF Ning Fu-Long Zhang Ke-Ni Wu Neng-You Jiang Guo-Sheng Zhang Ling Liu Li Yu Yi-Bing TI Invasion of water-based drilling mud into oceanic gas-hydrate-bearing sediment: One-dimensional numerical simulations SO CHINESE JOURNAL OF GEOPHYSICS-CHINESE EDITION LA Chinese DT Article DE Gas hydrate; Drilling fluid; Invasion; Hydrate dissociation; Secondary hydrate; Wellbore stability; Well logging ID GULF-OF-MEXICO; SATURATED UNCONSOLIDATED SEDIMENTS; CONTINENTAL-SLOPE; RELATIVE PERMEABILITY; METHANE HYDRATE; DEEP-WATER; WELL LOGS; MARINE; DEPOSITS; ACCUMULATIONS AB Integrating 3D seismic survey and well logging can achieve more accurate quantification of natural gas hydrates as a potential energy and environmental impact. However, some factors can influence the accurate interpretation and evaluation of well logging results. Except washouts, the invasions of drilling fluid probably also seriously distorts the results of well logging. In this work, we performed numerical simulations to study the dynamic behavior and general rules of mud invasion into oceanic gas hydrate bearing sediments (GHBS) by taking hydrate reservoirs in the Gulf of Mexico as a case. Compared with the conventional oil/gas-bearing sediments, hydrate dissociation and reformation are the main characteristics of mud invasion in GHBS when the invasion condition is in an unstable region of gas hydrates phase diagram. The simulation results show that the density (i. e., corresponding pressure), temperature, and salt content of drilling fluids have great effects on the process of drilling fluid invasion. When the temperature and salt content of drilling fluids are constants, the higher the density of the drilling fluid is, the greater degree of invasion and hydrate dissociation are. The increased pore pressure caused by the mud invasion, endothermic cooling with hydrate dissociation compounded by the Joule-Thompson effect and lagged effect of heat transfer in sediments, together make water and gas forming secondary hydrates. The secondary hydrate together with existing hydrate probably makes the hydrate saturation higher than original hydrate saturation. This high saturation hydrate ring could be attributed to the displacement effect of mud invasion and the permeability reduction because of secondary hydrates forming. Under the same temperature and pressure of drilling fluids, the higher the salt concentration of the drilling fluid, the faster rate and greater degree of hydrate dissociation due to the stronger thermodynamic inhibition effect and heat transfer efficiency. The occurrence of high-saturation hydrate girdle band seems to mainly depend on the temperature and salinity of drilling fluids. The dissociated free gas, the dilution of water salinity associated with hydrate dissociation and the occurrence of high saturation hydrate ring probably cause the calculated hydrate saturation based on well logging is higher than that of actual hydrate-bearing sediments. Our simulations suggest that in order to keep wellbore stability and well logging accuracy during drilling through the hydrate-bearing sediment, it is better to adopt the managed pressure drilling and low-temperature mud circulation, and add kinetic inhibitors or anti-agglomerants instead of salts into drilling fluids for preventing hydrate re-formation in the well. C1 [Ning Fu-Long; Jiang Guo-Sheng; Zhang Ling; Liu Li; Yu Yi-Bing] China Univ Geosci, Fac Engn, Wuhan 430074, Peoples R China. [Zhang Ke-Ni] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Earth Syst Div, Berkeley, CA 94720 USA. [Zhang Ke-Ni] Beijing Normal Univ, Coll Water Sci, Beijing 100875, Peoples R China. [Ning Fu-Long; Wu Neng-You] Chinese Acad Sci, Guangzhou Ctr Gas Hydrate Res, Guangzhou 510640, Peoples R China. RP Ning, FL (reprint author), China Univ Geosci, Fac Engn, Wuhan 430074, Peoples R China. EM nflzx@cug.edu.cn RI Ning, Fulong/G-4478-2010 OI Ning, Fulong/0000-0003-1236-586X NR 73 TC 1 Z9 8 U1 10 U2 42 PU SCIENCE PRESS PI BEIJING PA 16 DONGHUANGCHENGGEN NORTH ST, BEIJING 100717, PEOPLES R CHINA SN 0001-5733 J9 CHINESE J GEOPHYS-CH JI Chinese J. Geophys.-Chinese Ed. PD JAN PY 2013 VL 56 IS 1 BP 204 EP 218 DI 10.6038/cjg20130121 PG 15 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA 083QK UT WOS:000314480100021 ER PT J AU Leng, W Ju, L Gunzburger, M Price, S AF Leng, W. Ju, L. Gunzburger, M. Price, S. TI Manufactured solutions and the verification of three-dimensional Stokes ice-sheet models SO CRYOSPHERE LA English DT Article ID HIGHER-ORDER; BENCHMARK EXPERIMENTS; FLOW MODELS; ISMIP-HOM; APPROXIMATION; DYNAMICS AB The manufactured solution technique is used for the verification of computational models in many fields. In this paper, we construct manufactured solutions for the three-dimensional, isothermal, nonlinear Stokes model for flows in glaciers and ice sheets. The solution construction procedure starts with kinematic boundary conditions and is mainly based on the solution of a first-order partial differential equation for the ice velocity that satisfies the incompressibility condition. The manufactured solutions depend on the geometry of the ice sheet, basal sliding parameters, and ice softness. Initial conditions are taken from the periodic geometry of a standard problem of the ISMIP-HOM benchmark tests. The upper surface is altered through the manufactured solution procedure to generate an analytic solution for the time-dependent flow problem. We then use this manufactured solution to verify a parallel, high-order accurate, finite element Stokes ice-sheet model. Simulation results from the computational model show good convergence to the manufactured analytic solution. C1 [Leng, W.] Chinese Acad Sci, State Key Lab Sci & Engn Comp, Beijing 100190, Peoples R China. [Ju, L.] Univ S Carolina, Dept Math, Columbia, SC 29208 USA. [Ju, L.] Beijing Computat Sci Res Ctr, Beijing 100084, Peoples R China. [Gunzburger, M.] Florida State Univ, Dept Comp Sci, Tallahassee, FL 32306 USA. [Price, S.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Ju, L (reprint author), Univ S Carolina, Dept Math, Columbia, SC 29208 USA. EM ju@math.sc.edu; gunzburg@fsu.edu RI Price, Stephen /E-1568-2013 OI Price, Stephen /0000-0001-6878-2553 FU US Department of Energy, Office of Science, Advanced Scientific Computing Research and Biological and Environmental Research programs [DE-FG02-07ER64431, DE-FG02-07ER64432, DOE 07SCPF152]; Scientific Discovery through Advanced Computing (SciDAC) project "PISCEES"; US National Science Foundation [DMS-1215659] FX This work was partially supported by the US Department of Energy, Office of Science, Advanced Scientific Computing Research and Biological and Environmental Research programs through DE-FG02-07ER64431, DE-FG02-07ER64432, DOE 07SCPF152, and the Scientific Discovery through Advanced Computing (SciDAC) project "PISCEES", and by the US National Science Foundation under the grant number DMS-1215659. We also would like to thank the referees and the editor for their insightful comments which led to substantial improvements in the paper. NR 18 TC 11 Z9 11 U1 0 U2 13 PU COPERNICUS GESELLSCHAFT MBH PI GOTTINGEN PA BAHNHOFSALLEE 1E, GOTTINGEN, 37081, GERMANY SN 1994-0416 EI 1994-0424 J9 CRYOSPHERE JI Cryosphere PY 2013 VL 7 IS 1 BP 19 EP 29 DI 10.5194/tc-7-19-2013 PG 11 WC Geography, Physical; Geosciences, Multidisciplinary SC Physical Geography; Geology GA 087YK UT WOS:000314800400002 ER PT J AU Vasyukov, VA Glybin, AM Duday, PV Dudin, VI Zimenkov, AA Ivanov, VA Ivanovskiy, AV Kraev, AI Kuzyaev, AI Nadezhin, SS Petrukhin, AA Skobelev, AN Tyupanova, OA Atchison, WL Griego, JR Holtkamp, DB Kaul, AM Reinovsky, RE Rodriguez, G Tabaka, LJ Rousculp, CL Stone, JB Oro, DM Salazar, M Payton, JR Westley, DT AF Vasyukov, V. A. Glybin, A. M. Duday, P. V. Dudin, V. I. Zimenkov, A. A. Ivanov, V. A. Ivanovskiy, A. V. Kraev, A. I. Kuzyaev, A. I. Nadezhin, S. S. Petrukhin, A. A. Skobelev, A. N. Tyupanova, O. A. Atchison, W. L. Griego, J. R. Holtkamp, D. B. Kaul, A. M. Reinovsky, R. E. Rodriguez, G. Tabaka, L. J. Rousculp, C. L. Stone, J. B. Oro, D. M. Salazar, M. Payton, J. R. Westley, D. T. TI Rheology studies of aluminum with the use of explosive magnetic generators SO DOKLADY PHYSICS LA English DT Article C1 [Vasyukov, V. A.; Glybin, A. M.; Duday, P. V.; Dudin, V. I.; Zimenkov, A. A.; Ivanov, V. A.; Ivanovskiy, A. V.; Kraev, A. I.; Kuzyaev, A. I.; Nadezhin, S. S.; Petrukhin, A. A.; Skobelev, A. N.; Tyupanova, O. A.] All Russia Res Inst Expt Phys, Russian Fed Nucl Ctr, Sarov 607190, Russia. [Atchison, W. L.; Griego, J. R.; Holtkamp, D. B.; Kaul, A. M.; Reinovsky, R. E.; Rodriguez, G.; Tabaka, L. J.; Rousculp, C. L.; Stone, J. B.; Oro, D. M.; Salazar, M.; Payton, J. R.; Westley, D. T.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Vasyukov, VA (reprint author), All Russia Res Inst Expt Phys, Russian Fed Nucl Ctr, Sarov 607190, Russia. RI Rodriguez, George/G-7571-2012 OI Rodriguez, George/0000-0002-6044-9462 NR 12 TC 0 Z9 0 U1 0 U2 5 PU MAIK NAUKA/INTERPERIODICA/SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013-1578 USA SN 1028-3358 J9 DOKL PHYS JI Dokl. Phys. PD JAN PY 2013 VL 58 IS 1 BP 20 EP 23 DI 10.1134/S1028335813010096 PG 4 WC Mechanics; Physics, Multidisciplinary SC Mechanics; Physics GA 091GC UT WOS:000315036400005 ER PT J AU Wang, GS Post, WM Mayes, MA AF Wang, Gangsheng Post, Wilfred M. Mayes, Melanie A. TI Development of microbial-enzyme-mediated decomposition model parameters through steady-state and dynamic analyses SO ECOLOGICAL APPLICATIONS LA English DT Article DE decomposition; microbial biomass; multi-objective parameter sensitivity analysis (MOPSA); parameterization; soil enzymes ID DISSOLVED ORGANIC-CARBON; GREENHOUSE-GAS EMISSIONS; TERRESTRIAL ECOSYSTEMS; MANURE APPLICATIONS; THEORETICAL-MODEL; MINERAL SOILS; FOREST SOILS; MATTER; RESPIRATION; NITROGEN AB We developed a microbial-enzyme-mediated decomposition (MEND) model, based on the Michaelis-Menten kinetics, that describes the dynamics of physically defined pools of soil organic matter (SOC). These include particulate, mineral-associated, dissolved organic matter (POC, MOC, and DOC, respectively), microbial biomass, and associated exoenzymes. The ranges and/or distributions of parameters were determined by both analytical steady-state and dynamic analyses with SOC data from the literature. We used an improved multi-objective parameter sensitivity analysis (MOPSA) to identify the most important parameters for the full model: maintenance of microbial biomass, turnover and synthesis of enzymes, and carbon use efficiency (CUE). The model predicted that an increase of 2 degrees C (baseline temperature 12 degrees C) caused the pools of POC-cellulose, MOC, and total SOC to increase with dynamic CUE and decrease with constant CUE, as indicated by the 50% confidence intervals. Regardless of dynamic or constant CUE, the changes in pool size of POC, MOC, and total SOC varied from -8% to 8% under +2 degrees C. The scenario analysis using a single parameter set indicates that higher temperature with dynamic CUE might result in greater net increases in both POC-cellulose and MOC pools. Different dynamics of various SOC pools reflected the catalytic functions of specific enzymes targeting specific substrates and the interactions between microbes, enzymes, and SOC. With the feasible parameter values estimated in this study, models incorporating fundamental principles of microbial-enzyme dynamics can lead to simulation results qualitatively different from traditional models with fast/slow/passive pools. C1 [Wang, Gangsheng] Oak Ridge Natl Lab, Climate Change Sci Inst, Oak Ridge, TN 37831 USA. Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. RP Wang, GS (reprint author), Oak Ridge Natl Lab, Climate Change Sci Inst, Oak Ridge, TN 37831 USA. EM wangg@ornl.gov RI Wang, Gangsheng/F-8940-2012 OI Wang, Gangsheng/0000-0002-8117-5034 FU Laboratory Directed Research and Development Program of Oak Ridge National Laboratory; U.S. Department of Energy [DE-AC05-00OR22725] FX This research was sponsored by the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy under contract No. DE-AC05-00OR22725. The authors thank Xiaojuan Yang for her helpful comments. Thanks also go to the two anonymous reviewers for their constructive comments. This manuscript has been authored by UT-Battelle, LLC, under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains, and the publisher, by accepting the article for publication, acknowledges that the United States Government retains, a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. NR 67 TC 38 Z9 39 U1 7 U2 112 PU ECOLOGICAL SOC AMER PI WASHINGTON PA 1990 M STREET NW, STE 700, WASHINGTON, DC 20036 USA SN 1051-0761 J9 ECOL APPL JI Ecol. Appl. PD JAN PY 2013 VL 23 IS 1 BP 255 EP 272 PG 18 WC Ecology; Environmental Sciences SC Environmental Sciences & Ecology GA 092FM UT WOS:000315104800020 PM 23495650 ER PT J AU Belloni, F Calviani, M Colonna, N Mastinu, P Milazzo, PM Abbondanno, U Aerts, G Alvarez, H Alvarez-Velarde, F Andriamonje, S Andrzejewski, J Audouin, L Badurek, G Barbagallo, M Baumann, P Becvar, F Berthoumieux, E Calvino, F Cano-Ott, D Capote, R Carrapico, C Cennini, P Chepel, V Chiaveri, E Cortes, G Couture, A Cox, J Dahlfors, M David, S Dillmann, I Domingo-Pardo, C Dridi, W Duran, I Eleftheriadis, C Embid-Segura, M Ferrari, A Ferreira-Marques, R Fujii, K Furman, W Goncalves, I Gonzalez-Romero, E Goverdovski, A Gramegna, F Guerrero, C Gunsing, F Haas, B Haight, R Heil, M Herrera-Martinez, A Igashira, M Jericha, E Kappeler, F Kadi, Y Karadimos, D Karamanis, D Kerveno, M Koehler, P Kossionides, E Krticka, M Lamboudis, C Leeb, H Lindote, A Lopes, I Lozano, M Lukic, S Marganiec, J Marrone, S Martinez, T Massimi, C Meaze, MH Mengoni, A Moreau, C Mosconi, M Neves, F Oberhummer, H O'Brien, S Papachristodoulou, C Papadopoulos, C Paradela, C Patronis, N Pavlik, A Pavlopoulos, P Perrot, L Pigni, MT Plag, R Plompen, A Plukis, A Poch, A Praena, J Pretel, C Quesada, J Rauscher, T Reifarth, R Rosetti, M Rubbia, C Rudolf, G Rullhusen, P Salgado, J Santos, C Sarchiapone, L Savvidis, I Stephan, C Tagliente, G Tain, JL Tarrio, D Tassan-Got, L Tavora, L Terlizzi, R Vannini, G Vaz, P Ventura, A Villamarin, D Vincente, MC Vlachoudis, V Vlastou, R Voss, F Walter, S Wiescher, M Wisshak, K AF Belloni, F. Calviani, M. Colonna, N. Mastinu, P. Milazzo, P.-M. Abbondanno, U. Aerts, G. Alvarez, H. Alvarez-Velarde, F. Andriamonje, S. Andrzejewski, J. Audouin, L. Badurek, G. Barbagallo, M. Baumann, P. Becvar, F. Berthoumieux, E. Calvino, F. Cano-Ott, D. Capote, R. Carrapico, C. Cennini, P. Chepel, V. Chiaveri, E. Cortes, G. Couture, A. Cox, J. Dahlfors, M. David, S. Dillmann, I. Domingo-Pardo, C. Dridi, W. Duran, I. Eleftheriadis, C. Embid-Segura, M. Ferrari, A. Ferreira-Marques, R. Fujii, K. Furman, W. Goncalves, I. Gonzalez-Romero, E. Goverdovski, A. Gramegna, F. Guerrero, C. Gunsing, F. Haas, B. Haight, R. Heil, M. Herrera-Martinez, A. Igashira, M. Jericha, E. Kaeppeler, F. Kadi, Y. Karadimos, D. Karamanis, D. Kerveno, M. Koehler, P. Kossionides, E. Krticka, M. Lamboudis, C. Leeb, H. Lindote, A. Lopes, I. Lozano, M. Lukic, S. Marganiec, J. Marrone, S. Martinez, T. Massimi, C. Meaze, M.-H. Mengoni, A. Moreau, C. Mosconi, M. Neves, F. Oberhummer, H. O'Brien, S. Papachristodoulou, C. Papadopoulos, C. Paradela, C. Patronis, N. Pavlik, A. Pavlopoulos, P. Perrot, L. Pigni, M.-T. Plag, R. Plompen, A. Plukis, A. Poch, A. Praena, J. Pretel, C. Quesada, J. Rauscher, T. Reifarth, R. Rosetti, M. Rubbia, C. Rudolf, G. Rullhusen, P. Salgado, J. Santos, C. Sarchiapone, L. Savvidis, I. Stephan, C. Tagliente, G. Tain, J.-L. Tarrio, D. Tassan-Got, L. Tavora, L. Terlizzi, R. Vannini, G. Vaz, P. Ventura, A. Villamarin, D. Vincente, M.-C. Vlachoudis, V. Vlastou, R. Voss, F. Walter, S. Wiescher, M. Wisshak, K. TI Measurement of the neutron-induced fission cross-section of Am-241 at the time-of-flight facility n_TOF SO EUROPEAN PHYSICAL JOURNAL A LA English DT Article ID NUCLEAR-DATA; TECHNOLOGY; STANDARDS; FRAGMENTS; SCIENCE; SYSTEM; U-235; CERN AB The neutron-induced fission cross-section of Am-241 has been measured relative to the standard fission cross-section of U-235 between 0.5 and 20 MeV. The experiment was performed at the CERN n_TOF facility. Fission fragments were detected by a fast ionization chamber by discriminating against the alpha-particles from the high radioactivity of the samples. The high instantaneous neutron flux and the low background of the n_TOF facility enabled us to obtain uncertainties of approximate to 5%. With the present results it was possible to resolve discrepancies between previous data sets and to confirm current evaluations, thus providing important information for design studies of future reactors with improved fuel burn-up. C1 [Belloni, F.; Milazzo, P.-M.; Abbondanno, U.; Fujii, K.; Moreau, C.] Ist Nazl Fis Nucl INFN, Trieste, Italy. [Calviani, M.; Mastinu, P.; Gramegna, F.] Ist Nazl Fis Nucl, Lab Nazl Legnaro, Legnaro, Italy. [Calviani, M.; Cennini, P.; Chiaveri, E.; Dahlfors, M.; Ferrari, A.; Herrera-Martinez, A.; Kadi, Y.; Mengoni, A.; Sarchiapone, L.; Vlachoudis, V.] CERN, Geneva, Switzerland. [Colonna, N.; Barbagallo, M.; Marrone, S.; Meaze, M.-H.; Tagliente, G.; Terlizzi, R.] Ist Nazl Fis Nucl, Bari, Italy. [Aerts, G.; Andriamonje, S.; Berthoumieux, E.; Dridi, W.; Gunsing, F.; Perrot, L.; Plukis, A.] CEA, IRFU, Gif Sur Yvette, France. [Alvarez, H.; Cano-Ott, D.; Duran, I.; Embid-Segura, M.; Gonzalez-Romero, E.; Paradela, C.; Tarrio, D.] Univ Santiago Compostela, Santiago De Compostela, Spain. [Alvarez-Velarde, F.; Guerrero, C.; Martinez, T.; Villamarin, D.; Vincente, M.-C.] Ctr Invest Energet Medioambient & Technol, Madrid, Spain. [Andrzejewski, J.; Marganiec, J.] Univ Lodz, Lodz, Poland. [Audouin, L.; Dillmann, I.; Heil, M.; Kaeppeler, F.; Mosconi, M.; Plag, R.; Voss, F.; Walter, S.; Wisshak, K.] Karlsruhe Inst Technol, Inst Kernphys, Karlsruhe, Germany. [Badurek, G.; Jericha, E.; Leeb, H.; Oberhummer, H.] Vienna Univ Technol, Atominst Osterreich Univ, Vienna, Austria. [Baumann, P.; David, S.; Kerveno, M.; Lukic, S.; Rudolf, G.] Ctr Natl Rech Sci IN2P3 IReS, Strasbourg, France. [Becvar, F.; Krticka, M.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Calvino, F.; Cortes, G.; Poch, A.; Pretel, C.] Univ Politecn Cataluna, Barcelona, Spain. [Capote, R.; Mengoni, A.] Int Atomic Energy Agency IAEA, NAPC Nucl Data Sect, Vienna, Austria. [Capote, R.; Lozano, M.; Praena, J.; Quesada, J.] Univ Seville, Seville, Spain. [Carrapico, C.; Goncalves, I.; Salgado, J.; Santos, C.; Tavora, L.; Vaz, P.] Inst Tecnol & Nucl ITN, Lisbon, Portugal. [Chepel, V.; Ferreira-Marques, R.; Lindote, A.; Lopes, I.; Neves, F.] Univ Coimbra, LIP Coimbra, Dept Fis, Coimbra, Portugal. [Couture, A.; Cox, J.; O'Brien, S.; Wiescher, M.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Domingo-Pardo, C.; Tain, J.-L.] Univ Valencia, CSIC, Inst Fis Corpuscular, Valencia, Spain. [Eleftheriadis, C.; Lamboudis, C.; Savvidis, I.] Aristotle Univ Thessaloniki, Thessaloniki, Greece. [Furman, W.] Joint Inst Nucl Res, Frank Lab Neutron Phys, Dubna, Moscow Region, Russia. [Goverdovski, A.] Inst Phys & Power Engn, Obninsk, Russia. [Haas, B.] Ctr Natl Rech Sci IN2P3 CENBG, Bordeaux, France. [Haight, R.; Reifarth, R.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Igashira, M.] Tokyo Inst Technol, Tokyo, Japan. [Karadimos, D.; Karamanis, D.; Papachristodoulou, C.; Patronis, N.] Univ Ioannina, Ioannina, Greece. [Koehler, P.; Pigni, M.-T.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Kossionides, E.] NCSR, Athens, Greece. [Massimi, C.; Vannini, G.] Univ Bologna, Dipartimento Fis, Bologna, Italy. [Massimi, C.; Vannini, G.] Sezione Ist Nazl Fis Nucl, Bologna, Italy. [Papadopoulos, C.; Vlastou, R.] Natl Tech Univ Athens, Athens, Greece. [Pavlik, A.] Univ Vienna, Inst Fak Phys, Vienna, Austria. [Pavlopoulos, P.] Pole Univ Leonard Vinci, Paris, France. [Plompen, A.; Rullhusen, P.] CEC JRC IRMM, Geel, Belgium. [Rauscher, T.] Univ Basel, Dept Phys & Astron, Basel, Switzerland. [Rosetti, M.; Ventura, A.] ENEA, Bologna, Italy. [Rubbia, C.] Univ Pavia, Pavia, Italy. [Stephan, C.; Tassan-Got, L.] Ctr Natl Rech Sci IN2P3 IPN, Orsay, France. RP Belloni, F (reprint author), Ist Nazl Fis Nucl INFN, Trieste, Italy. EM paolo.milazzo@ts.infn.it RI Jericha, Erwin/A-4094-2011; Gonzalez Romero, Enrique/L-7561-2014; Pretel Sanchez, Carme/L-8287-2014; Martinez, Trinitario/K-6785-2014; Capote Noy, Roberto/M-1245-2014; Massimi, Cristian/B-2401-2015; Duran, Ignacio/H-7254-2015; Alvarez Pol, Hector/F-1930-2011; Massimi, Cristian/K-2008-2015; Paradela, Carlos/J-1492-2012; Gramegna, Fabiana/B-1377-2012; Calvino, Francisco/K-5743-2014; Mengoni, Alberto/I-1497-2012; Rauscher, Thomas/D-2086-2009; Quesada Molina, Jose Manuel/K-5267-2014; Guerrero, Carlos/L-3251-2014; Lozano, Manuel/L-6892-2014; Lindote, Alexandre/H-4437-2013; Neves, Francisco/H-4744-2013; Vaz, Pedro/K-2464-2013; Lopes, Isabel/A-1806-2014; Cortes, Guillem/B-6869-2014; Tain, Jose L./K-2492-2014; Cano Ott, Daniel/K-4945-2014 OI Lozano Leyva, Manuel Luis/0000-0003-2853-4103; Jericha, Erwin/0000-0002-8663-0526; Pavlik, Andreas/0000-0001-7526-3372; Goncalves, Isabel/0000-0002-1997-955X; Chepel, Vitaly/0000-0003-0675-4586; Marques, Rui/0000-0003-3549-8198; Domingo-Pardo, Cesar/0000-0002-2915-5466; Tarrio, Diego/0000-0002-9858-3341; Gonzalez Romero, Enrique/0000-0003-2376-8920; Martinez, Trinitario/0000-0002-0683-5506; Capote Noy, Roberto/0000-0002-1799-3438; Massimi, Cristian/0000-0001-9792-3722; Alvarez Pol, Hector/0000-0001-9643-6252; Massimi, Cristian/0000-0003-2499-5586; Gramegna, Fabiana/0000-0001-6112-0602; Calvino, Francisco/0000-0002-7198-4639; Mengoni, Alberto/0000-0002-2537-0038; Rauscher, Thomas/0000-0002-1266-0642; Quesada Molina, Jose Manuel/0000-0002-2038-2814; Guerrero, Carlos/0000-0002-2111-546X; Lindote, Alexandre/0000-0002-7965-807X; Neves, Francisco/0000-0003-3635-1083; Vaz, Pedro/0000-0002-7186-2359; Lopes, Isabel/0000-0003-0419-903X; Cano Ott, Daniel/0000-0002-9568-7508 FU EC [FIKW-CT-2000-00107]; European Union's Seventh Framework Programme under the ANDES project [249671] FX This work was supported by the EC under contract FIKW-CT-2000-00107 and by the funding agencies of the participating institutes. The research leading to these results has received funding from European Union's Seventh Framework Programme under the ANDES project, Grant Agreement n. 249671. NR 30 TC 5 Z9 5 U1 3 U2 43 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6001 J9 EUR PHYS J A JI Eur. Phys. J. A PD JAN PY 2013 VL 49 IS 1 AR 2 DI 10.1140/epja/i2013-13002-3 PG 6 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA 091KL UT WOS:000315048100002 ER PT J AU Park, K Guidal, M Gothe, RW Laget, JM Garcon, M Adhikari, KP Aghasyan, M Amaryan, MJ Anghinolfi, M Avakian, H Baghdasaryan, H Ball, J Baltzell, NA Battaglieri, M Bedlinsky, I Bennett, RP Biselli, AS Bookwalter, C Boiarinov, S Briscoe, WJ Brooks, WK Burkert, VD Carman, DS Celentano, A Chandavar, S Charles, G Contalbrigo, M Crede, V D'Angelo, A Daniel, A Dashyan, N De Vita, R De Sanctis, E Deur, A Djalali, C Dodge, GE Doughty, D Dupre, R Egiyan, H El Alaoui, A El Fassi, L Eugenio, P Fedotov, G Fegan, S Fleming, JA Forest, TA Fradi, A Gevorgyan, N Gilfoyle, GP Giovanetti, KL Girod, FX Gohn, W Golovatch, E Graham, L Griffioen, KA Guegan, B Guo, L Hafidi, K Hakobyan, H Hanretty, C Heddle, D Hicks, K Ho, D Holtrop, M Ilieva, Y Ireland, DG Ishkhanov, BS Jenkins, D Jo, HS Keller, D Khandaker, M Khetarpal, P Kim, A Kim, W Klein, FJ Koirala, S Kubarovsky, A Kubarovsky, V Kuhn, SE Kuleshov, SV Livingston, K Lu, HY MacGregor, IJD Mao, Y Markov, N Martinez, D Mayer, M McKinnon, B Meyer, CA Mineeva, T Mirazita, M Mokeev, V Moutarde, H Munevar, E Camacho, CM Nadel-Turonski, P Nepali, CS Niccolai, S Niculescu, G Niculescu, I Osipenko, M Ostrovidov, AI Pappalardo, LL Paremuzyan, R Park, S Pasyuk, E Pereira, SA Phelps, E Pisano, S Pogorelko, O Pozdniakov, S Price, JW Procureur, S Protopopescu, D Puckett, AJR Raue, BA Ricco, G Rimal, D Ripani, M Rosner, G Rossi, P Sabatie, F Saini, MS Salgado, C Schott, D Schumacher, RA Seder, E Seraydaryan, H Sharabian, YG Smith, ES Smith, GD Sober, DI Sokhan, D Stepanyan, SS Stoler, P Strakovsky, II Strauch, S Taiuti, M Tang, W Taylor, CE Tian, Y Tkachenko, S Trivedi, A Ungaro, M Vernarsky, B Voskanyan, H Voutier, E Walford, NK Watts, DP Weinstein, LB Weygand, DP Wood, MH Zachariou, N Zhang, J Zhao, ZW Zonta, I AF Park, K. Guidal, M. Gothe, R. W. Laget, J. M. Garcon, M. Adhikari, K. P. Aghasyan, M. Amaryan, M. J. Anghinolfi, M. Avakian, H. Baghdasaryan, H. Ball, J. Baltzell, N. A. Battaglieri, M. Bedlinsky, I. Bennett, R. P. Biselli, A. S. Bookwalter, C. Boiarinov, S. Briscoe, W. J. Brooks, W. K. Burkert, V. D. Carman, D. S. Celentano, A. Chandavar, S. Charles, G. Contalbrigo, M. Crede, V. D'Angelo, A. Daniel, A. Dashyan, N. De Vita, R. De Sanctis, E. Deur, A. Djalali, C. Dodge, G. E. Doughty, D. Dupre, R. Egiyan, H. El Alaoui, A. El Fassi, L. Eugenio, P. Fedotov, G. Fegan, S. Fleming, J. A. Forest, T. A. Fradi, A. Gevorgyan, N. Gilfoyle, G. P. Giovanetti, K. L. Girod, F. X. Gohn, W. Golovatch, E. Graham, L. Griffioen, K. A. Guegan, B. Guo, L. Hafidi, K. Hakobyan, H. Hanretty, C. Heddle, D. Hicks, K. Ho, D. Holtrop, M. Ilieva, Y. Ireland, D. G. Ishkhanov, B. S. Jenkins, D. Jo, H. S. Keller, D. Khandaker, M. Khetarpal, P. Kim, A. Kim, W. Klein, F. J. Koirala, S. Kubarovsky, A. Kubarovsky, V. Kuhn, S. E. Kuleshov, S. V. Livingston, K. Lu, H. Y. MacGregor, I. J. D. Mao, Y. Markov, N. Martinez, D. Mayer, M. McKinnon, B. Meyer, C. A. Mineeva, T. Mirazita, M. Mokeev, V. Moutarde, H. Munevar, E. Camacho, C. Munoz Nadel-Turonski, P. Nepali, C. S. Niccolai, S. Niculescu, G. Niculescu, I. Osipenko, M. Ostrovidov, A. I. Pappalardo, L. L. Paremuzyan, R. Park, S. Pasyuk, E. Pereira, S. Anefalos Phelps, E. Pisano, S. Pogorelko, O. Pozdniakov, S. Price, J. W. Procureur, S. Protopopescu, D. Puckett, A. J. R. Raue, B. A. Ricco, G. Rimal, D. Ripani, M. Rosner, G. Rossi, P. Sabatie, F. Saini, M. S. Salgado, C. Schott, D. Schumacher, R. A. Seder, E. Seraydaryan, H. Sharabian, Y. G. Smith, E. S. Smith, G. D. Sober, D. I. Sokhan, D. Stepanyan, S. S. Stoler, P. Strakovsky, I. I. Strauch, S. Taiuti, M. Tang, W. Taylor, C. E. Tian, Ye Tkachenko, S. Trivedi, A. Ungaro, M. Vernarsky, B. Voskanyan, H. Voutier, E. Walford, N. K. Watts, D. P. Weinstein, L. B. Weygand, D. P. Wood, M. H. Zachariou, N. Zhang, J. Zhao, Z. W. Zonta, I. TI Deep exclusive pi(+) electroproduction off the proton at CLAS SO EUROPEAN PHYSICAL JOURNAL A LA English DT Article ID VIRTUAL COMPTON-SCATTERING; PION FORM-FACTOR; CROSS-SECTION; HIGH-ENERGIES; SCALING LAWS; PHOTOPRODUCTION; DEUTERON; MESONS; PHOTODISINTEGRATION; MOMENTUM AB The exclusive electroproduction of pi(+) above the resonance region was studied using the CEBAF Large Acceptance Spectrometer (CLAS) at Jefferson Laboratory by scattering a 6 GeV continuous electron beam off a hydrogen target. The large acceptance and good resolution of CLAS, together with the high luminosity, allowed us to measure the cross section for the gamma*p -> n pi(+) process in 140 (Q(2), x(B), t) bins: 0.16 < x(B) < 0.58, 1.6 GeV2 < Q(2) < 4.5 GeV2 and 0.1 GeV2 < -t < 5.3 GeV2. For most bins, the statistical accuracy is on the order of a few percent. Differential cross sections are compared to four theoretical models, based either on hadronic or on partonic degrees of freedom. The four models can describe the gross features of the data reasonably well, but differ strongly in their ingredients. In particular, the model based on Generalized Parton Distributions (GPDs) contain the interesting potential to experimentally access transversity GPDs. C1 [Baltzell, N. A.; El Alaoui, A.; El Fassi, L.; Hafidi, K.] Argonne Natl Lab, Argonne, IL 60439 USA. [Pasyuk, E.] Arizona State Univ, Tempe, AZ 85287 USA. [Price, J. W.] Calif State Univ Dominguez Hills, Carson, CA 90747 USA. [Wood, M. H.] Canisius Coll, Buffalo, NY 14208 USA. [Ho, D.; Lu, H. Y.; Meyer, C. A.; Schumacher, R. A.; Vernarsky, B.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Klein, F. J.; Sober, D. I.; Walford, N. K.] Catholic Univ Amer, Washington, DC 20064 USA. [Garcon, M.; Ball, J.; Charles, G.; Dupre, R.; Moutarde, H.; Procureur, S.; Sabatie, F.] CEA, Ctr Saclay, Irfu, Serv Phys Nucl, F-91191 Gif Sur Yvette, France. [Doughty, D.; Heddle, D.] Christopher Newport Univ, Newport News, VA 23606 USA. [Gohn, W.; Markov, N.; Mineeva, T.; Seder, E.] Univ Connecticut, Storrs, CT 06269 USA. [Fleming, J. A.; Watts, D. P.] Univ Edinburgh, Edinburgh EH9 3JZ, Midlothian, Scotland. [Biselli, A. S.] Fairfield Univ, Fairfield, CT 06824 USA. [Guo, L.; Khetarpal, P.; Raue, B. A.; Rimal, D.; Schott, D.] Florida Int Univ, Miami, FL 33199 USA. [Bookwalter, C.; Crede, V.; Eugenio, P.; Ostrovidov, A. I.; Park, S.; Saini, M. S.] Florida State Univ, Tallahassee, FL 32306 USA. [Ricco, G.; Taiuti, M.] Univ Genoa, I-16146 Genoa, Italy. [Briscoe, W. J.; Ilieva, Y.; Niccolai, S.; Strakovsky, I. I.; Strauch, S.] George Washington Univ, Washington, DC 20052 USA. [Forest, T. A.; Martinez, D.; Taylor, C. E.] Idaho State Univ, Pocatello, ID 83209 USA. [Contalbrigo, M.; Pappalardo, L. L.] Ist Nazl Fis Nucl, Sez Ferrara, I-44100 Ferrara, Italy. [Aghasyan, M.; De Sanctis, E.; Mirazita, M.; Pereira, S. Anefalos; Pisano, S.; Rossi, P.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Anghinolfi, M.; Battaglieri, M.; Celentano, A.; De Vita, R.; Osipenko, M.; Ripani, M.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [D'Angelo, A.; Zonta, I.] INFN, Sez Roma Tor Vergata, I-00133 Rome, Italy. [Guidal, M.; Fradi, A.; Guegan, B.; Jo, H. S.; Camacho, C. Munoz; Niccolai, S.; Sokhan, D.] Inst Phys Nucl ORSAY, Orsay, France. [Bedlinsky, I.; Kuleshov, S. V.; Pogorelko, O.; Pozdniakov, S.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Giovanetti, K. L.; Niculescu, G.; Niculescu, I.] James Madison Univ, Harrisonburg, VA 22807 USA. [Kim, A.; Kim, W.; Stepanyan, S. S.] Kyungpook Natl Univ, Taegu 702701, South Korea. [Voutier, E.] Univ Grenoble 1, CNRS, IN2P3, LPSC,INPG, Grenoble, France. [Holtrop, M.; Protopopescu, D.] Univ New Hampshire, Durham, NH 03824 USA. [Khandaker, M.; Salgado, C.] Norfolk State Univ, Norfolk, VA 23504 USA. [Chandavar, S.; Daniel, A.; Hicks, K.; Niculescu, G.; Tang, W.] Ohio Univ, Athens, OH 45701 USA. [Adhikari, K. P.; Amaryan, M. J.; Bennett, R. P.; Dodge, G. E.; Koirala, S.; Kuhn, S. E.; Mayer, M.; Nepali, C. S.; Seraydaryan, H.; Weinstein, L. B.; Zhang, J.] Old Dominion Univ, Norfolk, VA 23529 USA. [Biselli, A. S.; Kubarovsky, A.; Stoler, P.; Ungaro, M.] Rensselaer Polytech Inst, Troy, NY 12180 USA. [Gilfoyle, G. P.] Univ Richmond, Richmond, VA 23173 USA. [D'Angelo, A.] Univ Roma Tor Vergata, I-00133 Rome, Italy. [Golovatch, E.; Ishkhanov, B. S.; Kubarovsky, A.; Mokeev, V.] Skobeltsyn Nucl Phys Inst, Moscow 119899, Russia. [Gothe, R. W.; Djalali, C.; Fedotov, G.; Graham, L.; Ilieva, Y.; Mao, Y.; Phelps, E.; Strauch, S.; Tian, Ye; Trivedi, A.; Wood, M. H.; Zachariou, N.] Univ S Carolina, Columbia, SC 29208 USA. [Park, K.; Laget, J. M.; Avakian, H.; Boiarinov, S.; Brooks, W. K.; Burkert, V. D.; Carman, D. S.; Deur, A.; Doughty, D.; Egiyan, H.; Girod, F. X.; Guo, L.; Heddle, D.; Kubarovsky, V.; Mokeev, V.; Munevar, E.; Nadel-Turonski, P.; Niculescu, I.; Pasyuk, E.; Puckett, A. J. R.; Raue, B. A.; Sharabian, Y. G.; Smith, E. S.; Ungaro, M.; Weygand, D. P.; Zhang, J.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. [Brooks, W. K.; Hakobyan, H.; Kuleshov, S. V.] Univ Tecn Federico Santa Maria, Valparaiso, Chile. [Fegan, S.; Ireland, D. G.; Livingston, K.; MacGregor, I. J. D.; McKinnon, B.; Protopopescu, D.; Rosner, G.; Smith, G. D.] Univ Glasgow, Glasgow G12 8QQ, Lanark, Scotland. [Jenkins, D.] Virginia Polytech Inst & State Univ, Blacksburg, VA 24061 USA. [Baghdasaryan, H.; Hanretty, C.; Keller, D.; Tkachenko, S.; Zhao, Z. W.] Univ Virginia, Charlottesville, VA 22901 USA. [Griffioen, K. A.] Coll William & Mary, Williamsburg, VA 23187 USA. [Baghdasaryan, H.; Dashyan, N.; Gevorgyan, N.; Hakobyan, H.; Paremuzyan, R.; Voskanyan, H.] Yerevan Phys Inst, Yerevan 375036, Armenia. RP Park, K (reprint author), Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. EM parkkj@jlab.org RI Zhang, Jixie/A-1461-2016; Celentano, Andrea/J-6190-2012; Osipenko, Mikhail/N-8292-2015; MacGregor, Ian/D-4072-2011; Brooks, William/C-8636-2013; Kuleshov, Sergey/D-9940-2013; Schumacher, Reinhard/K-6455-2013; Ishkhanov, Boris/E-1431-2012; Ireland, David/E-8618-2010; D'Angelo, Annalisa/A-2439-2012; Meyer, Curtis/L-3488-2014; Lu, Haiyun/B-4083-2012; Charles, Gabriel/B-7573-2015; El Alaoui, Ahmed/B-4638-2015; Sabatie, Franck/K-9066-2015 OI Celentano, Andrea/0000-0002-7104-2983; Zonta, Irene/0000-0003-4952-2160; Osipenko, Mikhail/0000-0001-9618-3013; Brooks, William/0000-0001-6161-3570; Kuleshov, Sergey/0000-0002-3065-326X; Schumacher, Reinhard/0000-0002-3860-1827; Ireland, David/0000-0001-7713-7011; D'Angelo, Annalisa/0000-0003-3050-4907; Meyer, Curtis/0000-0001-7599-3973; Sabatie, Franck/0000-0001-7031-3975 FU US Department of Energy; National Science Foundation; Italian Istituto Nazionale di Fisica Nucleare; French American Cultural Exchange (FACE); Partner University Funds (PUF) programs; French Centre National de la Recherche Scientifique; French Commissariat a l'Energie Atomique; United Kingdom's Science and Technology Facilities Council; Chilean Comision Nacional de Investigacion Cientifica y Tecnologica (CONICYT); National Research Foundation of Korea; US Department of Energy [DE-AC05-84ER40150] FX We acknowledge the outstanding efforts of the staff of the Accelerator and the Physics Divisions at Jefferson Lab that made this experiment possible. We also give many thanks to P. Kroll, S. Goloskokov and M. Kaskulov for their calculations. The early work of D. Dore on this analysis is also acknowledged. This work was supported in part by the US Department of Energy, the National Science Foundation, the Italian Istituto Nazionale di Fisica Nucleare, the French American Cultural Exchange (FACE) and Partner University Funds (PUF) programs, the French Centre National de la Recherche Scientifique, the French Commissariat a l'Energie Atomique, the United Kingdom's Science and Technology Facilities Council, the Chilean Comision Nacional de Investigacion Cientifica y Tecnologica (CONICYT), and the National Research Foundation of Korea. The Southeastern Universities Research Association (SURA) operated the Thomas Jefferson National Accelerator Facility for the US Department of Energy under Contract No. DE-AC05-84ER40150. NR 50 TC 7 Z9 7 U1 0 U2 23 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6001 J9 EUR PHYS J A JI Eur. Phys. J. A PD JAN PY 2013 VL 49 IS 1 AR 16 DI 10.1140/epja/i2013-13016-9 PG 18 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA 091KL UT WOS:000315048100016 ER PT J AU Gray, SB Strellner, RS Puthuval, KK Ng, C Shulman, RE Siebers, MH Rogers, A Leakey, ADB AF Gray, Sharon B. Strellner, Reid S. Puthuval, Kannan K. Ng, Christopher Shulman, Ross E. Siebers, Matthew H. Rogers, Alistair Leakey, Andrew D. B. TI Minirhizotron imaging reveals that nodulation of field-grown soybean is enhanced by free-air CO2 enrichment only when combined with drought stress SO FUNCTIONAL PLANT BIOLOGY LA English DT Article DE elevated CO2; FACE; Glycine max; nodule; root ID ELEVATED ATMOSPHERIC CO2; CARBON-DIOXIDE CONCENTRATION; SYMBIOTIC NITROGEN-FIXATION; N-2 FIXATION; NODULE DISTRIBUTION; N-2-FIXING ALFALFA; SOIL-MOISTURE; CORN-BELT; LEGUME; PHOTOSYNTHESIS AB The rate of N-2 fixation by a leguminous plant is a product of the activity of individual nodules and the number of nodules. Initiation of new nodules and N-2 fixation per nodule are highly sensitive to environmental conditions. However, the effects of global environmental change on nodulation in the field are largely unknown. It is also unclear whether legumes regulate nodulation in response to environment solely by varying root production or also by varying nodule density per unit of root length. This study utilised minirhizotron imaging as a novel in situ method for assessing the number, size and distribution of nodules in field-grown soybean (Glycine max (L.) Merr.) exposed to elevated atmospheric CO2 ([CO2]) and reduced precipitation. We found that nodule numbers were 134-229% greater in soybeans grown at elevated [CO2] in combination with reduced precipitation, and this response was driven by greater nodule density per unit of root length. The benefits of additional nodules were probably offset by an unfavourable distribution of nodules in shallow, dry soil in reduced precipitation treatment under elevated [CO2] but not ambient [CO2]. In fact, significant decreases in seed and leaf nitrogen concentration also occurred only in elevated [CO2] with reduced precipitation. This study demonstrates the potential of minirhizotron imaging to reveal previously uncharacterised changes in nodule production and distribution in response to global environmental change. C1 [Gray, Sharon B.; Strellner, Reid S.; Puthuval, Kannan K.; Ng, Christopher; Siebers, Matthew H.; Leakey, Andrew D. B.] Univ Illinois, Dept Plant Biol, Inst Genom Biol, Urbana, IL 61801 USA. [Shulman, Ross E.; Rogers, Alistair] Brookhaven Natl Lab, Dept Environm Sci, Upton, NY 11973 USA. RP Leakey, ADB (reprint author), Univ Illinois, Dept Plant Biol, Inst Genom Biol, 1206 W Gregory Dr, Urbana, IL 61801 USA. EM leakey@illinois.edu RI Rogers, Alistair/E-1177-2011; Leakey, Andrew/Q-9889-2016 OI Rogers, Alistair/0000-0001-9262-7430; Leakey, Andrew/0000-0001-6251-024X FU USA Department of Agriculture Agricultural Research Service; Department of Energy through the Office of Science Midwestern Regional Center of the National Institute for Climatic Change Research at Michigan Technological University [DE-FC02-06ER64158]; National Research Initiative of Agriculture and Food Research Initiative Competitive Grants Program [2010-65114-20343]; USDA National Institute of Food and Agriculture [DE-AC02-98CH10886]; DOE Global Change Education Program Graduate Research on the Environment Fellowship; Beckman Fellowship from the Center for Advanced Studies, University of Illinois at Urbana-Champaign (UIUC); Environmental Change Institute, UIUC FX We thank the following people for invaluable assistance with sample collection and field site maintenance and operations: Lorena Rios Acosta, Elizabeth Ainsworth, Carl Bernacchi, Amy Betzelberger, Chris Black, Geoff Boise, Ryan Boyd, Phil Brandyberry, Christina Burke, Sarah Campbell, Nathan Couch, David Drag, Alex Hargus, Doug Klier, Bob Koester, Courtney Leisner, Anna Locke, Cody Markelz, Chris Montes, Don Ort, Katie Richter, David Rosenthal, Mike Suguitan, Becky Slattery, Joe Sullivan, Brianna Usdrowski, Ursula Ruiz Vera and Adrian Zimbelman. The SoyFACE facility was supported by the USA Department of Agriculture Agricultural Research Service. This project was, in part, supported by Department of Energy through the Office of Science Midwestern Regional Center of the National Institute for Climatic Change Research at Michigan Technological University under Award Number DE-FC02-06ER64158, the National Research Initiative of Agriculture and Food Research Initiative Competitive Grants Program Grant No. 2010-65114-20343 from the USDA National Institute of Food and Agriculture, and through Contract No. DE-AC02-98CH10886 to Brookhaven National Laboratory. SBG was supported by the DOE Global Change Education Program Graduate Research on the Environment Fellowship. ADBL was supported by a Beckman Fellowship from the Center for Advanced Studies, University of Illinois at Urbana-Champaign (UIUC), and a Fellowship from the Environmental Change Institute, UIUC. NR 53 TC 8 Z9 9 U1 1 U2 73 PU CSIRO PUBLISHING PI COLLINGWOOD PA 150 OXFORD ST, PO BOX 1139, COLLINGWOOD, VICTORIA 3066, AUSTRALIA SN 1445-4408 J9 FUNCT PLANT BIOL JI Funct. Plant Biol. PY 2013 VL 40 IS 2 SI SI BP 137 EP 147 DI 10.1071/FP12044 PG 11 WC Plant Sciences SC Plant Sciences GA 089GS UT WOS:000314899600005 ER PT J AU Zortman, WA Lentine, AL Trotter, DC Watts, MR AF Zortman, William A. Lentine, Anthony L. Trotter, Douglas C. Watts, Michael R. TI BIT-ERROR-RATE MONITORING FOR ACTIVE WAVELENGTH CONTROL OF RESONANT MODULATORS SO IEEE MICRO LA English DT Article ID SILICON ELECTROOPTIC MODULATOR; INTEGRATION AB A new method uses bit-error-rate measurements to acquire and stabilize the wavelength of an optical resonant modulator to an optical carrier wave. This is attractive because it uses the pertinent metric, bit error rate, to optimize the modulator resonance independent of other system variations, meaning it can compensate for system aging and drift even in the heater element itself. C1 [Zortman, William A.] Sandia Natl Labs, Appl Photon Microsyst Grp, Albuquerque, NM 87123 USA. [Lentine, Anthony L.] Sandia Natl Labs, Tech Staff, Albuquerque, NM 87123 USA. [Trotter, Douglas C.] Sandia Natl Labs, Albuquerque, NM 87123 USA. [Watts, Michael R.] MIT, Elect Engn & Comp Sci Dept, Cambridge, MA 02139 USA. RP Zortman, WA (reprint author), Sandia Natl Labs, Appl Photon Microsyst Grp, 1515 Eubank Blvd,MS 1082, Albuquerque, NM 87123 USA. EM wzortm@sandia.gov FU US Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia, a wholly owned subsidiary of Lockheed Martin, for the US Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 18 TC 22 Z9 22 U1 0 U2 2 PU IEEE COMPUTER SOC PI LOS ALAMITOS PA 10662 LOS VAQUEROS CIRCLE, PO BOX 3014, LOS ALAMITOS, CA 90720-1314 USA SN 0272-1732 EI 1937-4143 J9 IEEE MICRO JI IEEE Micro PD JAN-FEB PY 2013 VL 33 IS 1 BP 42 EP 52 PG 11 WC Computer Science, Hardware & Architecture; Computer Science, Software Engineering SC Computer Science GA 090VF UT WOS:000315007400007 ER PT J AU Ning, PQ Wang, F Ngo, KDT AF Ning, Puqi Wang, Fei (Fred) Ngo, Khai D. T. TI Automatic Layout Design for Power Module SO IEEE TRANSACTIONS ON POWER ELECTRONICS LA English DT Article DE Layout; packaging ID PERFORMANCE; DIODE AB The layout of power modules is one of the key points in power module design, especially for high power densities, where couplings are increased. In this paper, along with the design example, automatic design processes by using a genetic algorithm are presented. Some practical considerations and implementations are introduced in the optimization of module layout design. C1 [Ning, Puqi; Wang, Fei (Fred)] Oak Ridge Natl Lab, Natl Transportat Res Ctr, Knoxville, TN 37932 USA. [Wang, Fei (Fred)] Univ Tennessee, Dept Elect Engn & Comp Sci, Knoxville, TN 37996 USA. [Ngo, Khai D. T.] Virginia Polytech Inst & State Univ, Ctr Power Elect Syst, Blacksburg, VA 24060 USA. RP Ning, PQ (reprint author), Oak Ridge Natl Lab, Natl Transportat Res Ctr, Knoxville, TN 37932 USA. EM ningp@ornl.gov FU UT-Battelle, LLC [DE-AC05-00OR22725]; U.S. Department of Energy; National Science Foundation [EEC-9731677] FX This work is supported by UT-Battelle, LLC, under Contract DE-AC05-00OR22725 with the U.S. Department of Energy. The U.S. government retains and the publisher, by accepting the article for publication, acknowledges that the United States government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for U.S. government purposes.; This paper made use of Engineering Research Center Shared Facilities supported by the National Science Foundation under Award EEC-9731677. The authors would like to acknowledge the help of Dr. Dushan Boroyevich from the Center for Power Electronics Systems, Virginia Polytechnic Institute and State University. NR 20 TC 6 Z9 6 U1 0 U2 10 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0885-8993 J9 IEEE T POWER ELECTR JI IEEE Trans. Power Electron. PD JAN PY 2013 VL 28 IS 1 BP 481 EP 487 DI 10.1109/TPEL.2011.2180739 PG 7 WC Engineering, Electrical & Electronic SC Engineering GA 086OK UT WOS:000314694500047 ER PT J AU Wang, RX Boroyevich, D Ning, PQ Wang, ZQ Wang, F Mattavelli, P Ngo, KDT Rajashekara, K AF Wang, Ruxi Boroyevich, Dushan Ning, Puqi Wang, Zhiqiang Wang, Fei Mattavelli, Paolo Ngo, Khai D. T. Rajashekara, Kaushik TI A High-Temperature SiC Three-Phase AC-DC Converter Design for > 100 degrees C Ambient Temperature SO IEEE TRANSACTIONS ON POWER ELECTRONICS LA English DT Article DE Harsh environment; high-temperature (HT) converter; silicon carbide JFET; silicon-on-insulator (SOI) technology ID POWER ELECTRONICS; MODULES; DEVICES; ENVIRONMENTS; INTEGRATION; OPERATION; JFET AB High-temperature (HT) converters have gained importance in industrial applications where the converters operate in a harsh environment, such as in hybrid electrical vehicles, aviation, and deep-earth petroleum exploration. These environments require the converter to have not only HT semiconductor devices (made of SiC or GaN), but also reliable HT packaging, HT gate drives, and HT control electronics. This paper describes a detailed design process for an HT SiC three-phase PWM rectifier that can operate at ambient temperatures above 100 degrees C. SiC HT planar structure packaging is designed for the main semiconductor devices, and an edge-triggeredHT gate drive is also proposed to drive the designed power module. The system is designed to make use of available HT components, including the passive components, silicon-on-insulator chips, and auxiliary components. Finally, a 1.4 kW lab prototype is tested in a harsh environment for verification. C1 [Wang, Ruxi; Boroyevich, Dushan; Mattavelli, Paolo; Ngo, Khai D. T.] Virginia Polytech Inst & State Univ, Dept Elect & Comp Engn, Ctr Power Elect Syst, Blacksburg, VA 24060 USA. [Ning, Puqi] Oak Ridge Natl Lab, Natl Transportat Res Ctr, Oak Ridge, TN 37831 USA. [Wang, Zhiqiang; Wang, Fei] Univ Tennessee, Knoxville, TN 37916 USA. [Wang, Fei] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Rajashekara, Kaushik] Rolls Royce Corp, Indianapolis, IN 46241 USA. RP Wang, RX (reprint author), Virginia Polytech Inst & State Univ, Dept Elect & Comp Engn, Ctr Power Elect Syst, Blacksburg, VA 24060 USA. EM ruxi@vt.edu; dushan@vt.edu; ning06@vt.edu; zqwang@vt.edu; fred.wang@utk.edu; mattavelli@ieee.org; kdtn@vt.edu; K.Rajashekara@Rolls-Royce.com FU Rolls-Royce Corporation FX This work was supported by the Rolls-Royce Corporation. Recommended for publication by Associate Editor E. Santi. NR 36 TC 45 Z9 48 U1 0 U2 22 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0885-8993 EI 1941-0107 J9 IEEE T POWER ELECTR JI IEEE Trans. Power Electron. PD JAN PY 2013 VL 28 IS 1 BP 555 EP 572 DI 10.1109/TPEL.2012.2199131 PG 18 WC Engineering, Electrical & Electronic SC Engineering GA 086OK UT WOS:000314694500055 ER PT J AU Alfeld, M De Nolf, W Cagno, S Appel, K Siddons, DP Kuczewski, A Janssens, K Dik, J Trentelman, K Walton, M Sartorius, A AF Alfeld, Matthias De Nolf, Wout Cagno, Simone Appel, Karen Siddons, D. Peter Kuczewski, Anthony Janssens, Koen Dik, Joris Trentelman, Karen Walton, Marc Sartorius, Andrea TI Revealing hidden paint layers in oil paintings by means of scanning macro-XRF: a mock-up study based on Rembrandt's "An old man in military costume" SO JOURNAL OF ANALYTICAL ATOMIC SPECTROMETRY LA English DT Article ID RAY; SPECTRA; SYSTEM; MICROPROBE; LIBRARY; OBJECTS; PIXE; ART AB Over the past several decades the oeuvre of Rembrandt has been the subject of extensive art historical and scientific investigations. One of the most striking features to emerge is his frequent re-use of canvases and panels. The painting An Old Man in Military Costume (78.PB.246), in the collection of the J. Paul Getty Museum, is an example of such a re-used panel. Conventional imaging techniques revealed the presence of a second portrait under the surface portrait, but the details of this hidden portrait have not yet been revealed. Vermilion (HgS) has been identified to have been used nearly exclusively in the flesh tones of the lower painting, suggesting that element-specific XRF imaging might successfully image the hidden portrait. To test this hypothesis, a full-scale mock-up of the painting was created, including a "free impression" of the hidden portrait, reproducing as closely as possible the pigments and paint stratigraphy of the original painting. XRF imaging of the mock-up painting was conducted using three different XRF imaging systems: a mobile X-ray tube based system and two synchrotron-based setups (one equipped with multiple SDDs and one equipped with a Maia detector). The sensitivity, limits of detection and imaging capabilities of each system under the chosen experimental conditions are evaluated and compared. The results indicate that an investigation of the original painting by this method would have an excellent chance of success. C1 [Alfeld, Matthias; De Nolf, Wout; Cagno, Simone; Janssens, Koen] Univ Antwerp, Dept Chem, AXI2L Res Grp, B-2020 Antwerp, Belgium. [Appel, Karen] Deutsch Elektronen Synchrotron DESY, Hamburger Synchrotronstrahlungslab HASYLAB, D-22607 Hamburg, Germany. [Siddons, D. Peter; Kuczewski, Anthony] Brookhaven Natl Lab, Natl Synchrotron Light Source, Upton, NY 11973 USA. [Dik, Joris] Delft Univ Technol, Dept Mat Sci, NL-2628 CD Delft, Netherlands. [Trentelman, Karen; Walton, Marc] Getty Conservat Inst, Los Angeles, CA 90049 USA. [Sartorius, Andrea] J Paul Getty Museum, Paintings Conservat Dept, Los Angeles, CA 90049 USA. RP Alfeld, M (reprint author), Univ Antwerp, Dept Chem, AXI2L Res Grp, Groenborgerlaan 171, B-2020 Antwerp, Belgium. EM matthias.alfeld@ua.ac.be; koen.janssens@ua.ac.be RI Janssens, Koen/B-8049-2011; Alfeld, Matthias/L-6748-2016; Cagno, Simone/A-6312-2017 OI Janssens, Koen/0000-0002-6752-6408; Alfeld, Matthias/0000-0001-7974-9564; Cagno, Simone/0000-0002-3860-6812 FU Interuniversity Attraction Poles Programme - Belgian Science Policy [IUAP VI/16]; Research Fund University of Antwerp, Belgium; FWO (Brussels, Belgium) [G.0704.08, G.01769.09]; European Community [226716]; Research Foundation - Flanders (FWO) FX This research was supported by the Interuniversity Attraction Poles Programme - Belgian Science Policy (IUAP VI/16). The text also presents results of GOA "XANES meets ELNES" (Research Fund University of Antwerp, Belgium) and from FWO (Brussels, Belgium) projects no. G.0704.08 and G.01769.09. Further, the research leading to these results has received funding from the European Community's Seventh Framework Programme (FP7/2007-2013) under grant agreement no 226716. M. Alfeld receives a Ph.D. fellowship of the Research Foundation - Flanders (FWO). The authors gratefully acknowledge Yvonne Szafran and the staff of the Paintings Conservation Department of the J. Paul Getty Museum for making available their infrared reflectography (IRR) and X-radiographic images of the painting, and also the neutron activation analysis (NAA) images acquired in 1996 at NIST by Dr Henry Prask in collaboration with Mark Leonard, former head of the J. Paul Getty Museum Paintings Conservation Department. We are also grateful to Peter Reischig, a graduate intern at the Getty Conservation Institute and a Ph.D. candidate at Delft University of Technology for his assistance. NR 25 TC 18 Z9 18 U1 2 U2 56 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 0267-9477 J9 J ANAL ATOM SPECTROM JI J. Anal. At. Spectrom. PD JAN PY 2013 VL 28 IS 1 BP 40 EP 51 DI 10.1039/c2ja30119a PG 12 WC Chemistry, Analytical; Spectroscopy SC Chemistry; Spectroscopy GA 089IE UT WOS:000314903400003 ER PT J AU Alessandria, F Ardito, R Artusa, DR Avignone, FT Azzolini, O Balata, M Banks, TI Bari, G Beeman, J Bellini, F Bersani, A Biassoni, M Bloxham, T Brofferio, C Bucci, C Cai, XZ Canonica, L Capelli, S Carbone, L Cardani, L Carrettoni, M Casali, N Chott, N Clemenza, M Cosmelli, C Cremonesi, O Creswick, RJ Dafinei, I Dally, A Datskov, V De Biasi, A Decowski, MP Deninno, MM Di Domizio, S di Vacri, ML Ejzak, L Faccini, R Fang, DQ Farach, HA Ferri, E Ferroni, F Fiorini, E Franceschi, MA Freedman, SJ Fujikawa, BK Giachero, A Gironi, L Giuliani, A Goett, J Gorla, P Gotti, C Guardincerri, E Gutierrez, TD Haller, EE Han, K Heeger, KM Huang, HZ Kadel, R Kazkaz, K Keppel, G Kogler, L Kolomensky, YG Lenz, D Li, YL Ligi, C Liu, X Ma, YG Maiano, C Maino, M Martinez, M Maruyama, RH Moggi, N Morganti, S Napolitano, T Newman, S Nisi, S Nones, C Norman, EB Nucciotti, A Orio, F Orlandi, D Ouellet, JL Pallavicini, M Palmieri, V Pattavina, L Pavan, M Pedretti, M Pessina, G Pirro, S Previtali, E Rampazzo, V Rimondi, F Rosenfeld, C Rusconi, C Sangiorgio, S Scielzo, ND Sisti, M Smith, AR Stivanello, F Taffarello, L Tenconi, M Tian, WD Tomei, C Trentalange, S Ventura, G Vignati, M Wang, BS Wang, HW Whitten, CA Wise, T Woodcraft, A Zanotti, L Zarra, C Zhu, BX Zucchelli, S AF Alessandria, F. Ardito, R. Artusa, D. R. Avignone, F. T., III Azzolini, O. Balata, M. Banks, T. I. Bari, G. Beeman, J. Bellini, F. Bersani, A. Biassoni, M. Bloxham, T. Brofferio, C. Bucci, C. Cai, X. Z. Canonica, L. Capelli, S. Carbone, L. Cardani, L. Carrettoni, M. Casali, N. Chott, N. Clemenza, M. Cosmelli, C. Cremonesi, O. Creswick, R. J. Dafinei, I. Dally, A. Datskov, V. De Biasi, A. Decowski, M. P. Deninno, M. M. Di Domizio, S. di Vacri, M. L. Ejzak, L. Faccini, R. Fang, D. Q. Farach, H. A. Ferri, E. Ferroni, F. Fiorini, E. Franceschi, M. A. Freedman, S. J. Fujikawa, B. K. Giachero, A. Gironi, L. Giuliani, A. Goett, J. Gorla, P. Gotti, C. Guardincerri, E. Gutierrez, T. D. Haller, E. E. Han, K. Heeger, K. M. Huang, H. Z. Kadel, R. Kazkaz, K. Keppel, G. Kogler, L. Kolomensky, Yu G. Lenz, D. Li, Y. L. Ligi, C. Liu, X. Ma, Y. G. Maiano, C. Maino, M. Martinez, M. Maruyama, R. H. Moggi, N. Morganti, S. Napolitano, T. Newman, S. Nisi, S. Nones, C. Norman, E. B. Nucciotti, A. Orio, F. Orlandi, D. Ouellet, J. L. Pallavicini, M. Palmieri, V. Pattavina, L. Pavan, M. Pedretti, M. Pessina, G. Pirro, S. Previtali, E. Rampazzo, V. Rimondi, F. Rosenfeld, C. Rusconi, C. Sangiorgio, S. Scielzo, N. D. Sisti, M. Smith, A. R. Stivanello, F. Taffarello, L. Tenconi, M. Tian, W. D. Tomei, C. Trentalange, S. Ventura, G. Vignati, M. Wang, B. S. Wang, H. W. Whitten, C. A., Jr. Wise, T. Woodcraft, A. Zanotti, L. Zarra, C. Zhu, B. X. Zucchelli, S. CA CUORE Collaboration TI The low energy spectrum of TeO2 bolometers: results and dark matter perspectives for the CUORE-0 and CUORE experiments SO JOURNAL OF COSMOLOGY AND ASTROPARTICLE PHYSICS LA English DT Article DE dark matter detectors; dark matter experiments ID INTERACTING MASSIVE PARTICLES; NUCLEAR-DATA SHEETS; RESPONSE STABILIZATION; CUORICINO; CANDIDATES; SEARCH; CONSTRAINTS; CONDUCTION; DETECTORS; SIGNALS AB We collected 19.4 days of data from four 750g TeO2 bolometers, and in three of them we were able to set the energy threshold around 3 keV using a new analysis technique. We found a background rate ranging from 25 cpd/keV/kg at 3 keV to 2 cpd/keV/kg at 25 keV, and a peak at 4.7 keV. The origin of this peak is presently unknown, but its presence is confirmed by a reanalysis of 62.7 kg.days of data from the finished CUORICINO experiment. Finally, we report the expected sensitivities of the CUORE-0 (52 bolometers) and CUORE (988 bolometers) experiments to a WIMP annual modulation signal. C1 [Alessandria, F.] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Ardito, R.] Politecn Milan, Dipartimento Ingn Strutturale, I-20133 Milan, Italy. [Artusa, D. R.; Avignone, F. T., III; Chott, N.; Creswick, R. J.; Farach, H. A.; Newman, S.; Rosenfeld, C.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Artusa, D. R.; Balata, M.; Banks, T. I.; Bucci, C.; Canonica, L.; Casali, N.; di Vacri, M. L.; Goett, J.; Guardincerri, E.; Newman, S.; Nisi, S.; Orlandi, D.; Zarra, C.] Ist Nazl Fis Nucl, Lab Nazl Gran Sasso, I-67010 Laquila, Italy. [Azzolini, O.; De Biasi, A.; Keppel, G.; Palmieri, V.; Rampazzo, V.; Stivanello, F.] Ist Nazl Fis Nucl, Lab Nazl Legnaro, I-35020 Padua, Italy. [Banks, T. I.; Decowski, M. P.; Freedman, S. J.; Kogler, L.; Kolomensky, Yu G.; Ouellet, J. L.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Banks, T. I.; Bloxham, T.; Decowski, M. P.; Deninno, M. M.; Freedman, S. J.; Fujikawa, B. K.; Guardincerri, E.; Han, K.; Kogler, L.; Ouellet, J. L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Bari, G.; Moggi, N.; Rimondi, F.; Zucchelli, S.] Ist Nazl Fis Nucl, Sez Bologna, I-40127 Bologna, Italy. [Beeman, J.; Haller, E. E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Bellini, F.; Cardani, L.; Cosmelli, C.; Faccini, R.; Ferroni, F.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Bellini, F.; Cardani, L.; Cosmelli, C.; Dafinei, I.; Faccini, R.; Ferroni, F.; Morganti, S.; Orio, F.; Tomei, C.; Vignati, M.] Ist Nazl Fis Nucl, Sez Roma, I-00185 Rome, Italy. [Bersani, A.; Di Domizio, S.; Pallavicini, M.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Biassoni, M.; Brofferio, C.; Capelli, S.; Carrettoni, M.; Clemenza, M.; Ferri, E.; Fiorini, E.; Gironi, L.; Gotti, C.; Maiano, C.; Maino, M.; Nucciotti, A.; Pavan, M.; Sisti, M.; Zanotti, L.] Univ Milano Bicocca, Dipartimento Fis, I-20126 Milan, Italy. [Biassoni, M.; Brofferio, C.; Capelli, S.; Carbone, L.; Carrettoni, M.; Clemenza, M.; Cremonesi, O.; Datskov, V.; Ferri, E.; Fiorini, E.; Giachero, A.; Gironi, L.; Gotti, C.; Maiano, C.; Maino, M.; Nucciotti, A.; Pattavina, L.; Pavan, M.; Pirro, S.; Previtali, E.; Rusconi, C.; Sisti, M.; Zanotti, L.] Ist Nazl Fis Nucl, Sez Milano Bicocca, I-20126 Milan, Italy. [Cai, X. Z.; Fang, D. Q.; Li, Y. L.; Ma, Y. G.; Tian, W. D.; Wang, H. W.] Chinese Acad Sci, Shanghai Inst Appl Phys, Shanghai 201800, Peoples R China. [Dally, A.; Ejzak, L.; Heeger, K. M.; Lenz, D.; Maruyama, R. H.; Wise, T.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Di Domizio, S.; Pallavicini, M.] Univ Genoa, Dipartimento Fis, I-16146 Genoa, Italy. [Franceschi, M. A.; Ligi, C.; Napolitano, T.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Roma, Italy. [Giuliani, A.; Tenconi, M.] Ctr Spectrometrie Nucl & Spectrometrie Masse, F-91405 Orsay, France. [Gorla, P.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, I-00133 Rome, Italy. [Gutierrez, T. D.] Calif Polytech State Univ San Luis Obispo, Dept Phys, San Luis Obispo, CA 93407 USA. [Haller, E. E.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Huang, H. Z.; Liu, X.; Trentalange, S.; Whitten, C. A., Jr.; Zhu, B. X.] Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA. [Kadel, R.; Kolomensky, Yu G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Kazkaz, K.; Norman, E. B.; Pedretti, M.; Pessina, G.; Sangiorgio, S.; Scielzo, N. D.; Wang, B. S.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Martinez, M.] Univ Zaragoza, Lab Fis Nucl & Astoparticulas, E-50009 Zaragoza, Spain. [Nones, C.] CEA Saclay, Serv Phys Particules, F-91191 Gif Sur Yvette, France. [Norman, E. B.; Wang, B. S.] Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA. [Rimondi, F.; Zucchelli, S.] Univ Bologna, Dipartmento Fis, I-40127 Bologna, Italy. [Smith, A. R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, EH&S Div, Berkeley, CA 94720 USA. [Taffarello, L.] Ist Nazl Fis Nucl, Sez Padova, I-35131 Padua, Italy. [Ventura, G.] Univ Florence, Dipartimento Fis, I-50125 Florence, Italy. [Ventura, G.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Woodcraft, A.] Univ Edinburgh, Inst Astron, SUPA, Edinburgh EH9 3HJ, Midlothian, Scotland. RP Alessandria, F (reprint author), Ist Nazl Fis Nucl, Sez Milano, Via Celoria 16, I-20133 Milan, Italy. RI Ligi, Carlo/M-4007-2016; Gironi, Luca/P-2860-2016; capelli, silvia/G-5168-2012; Ma, Yu-Gang/M-8122-2013; Casali, Nicola/C-9475-2017; Han, Ke/D-3697-2017; Vignati, Marco/H-1684-2013; Giachero, Andrea/I-1081-2013; Bellini, Fabio/D-1055-2009; Gorla, Paolo/B-5243-2014; Sangiorgio, Samuele/F-4389-2014; Nucciotti, Angelo/I-8888-2012; Martinez, Maria/K-4827-2012; Di Domizio, Sergio/L-6378-2014; Ferri, Elena/L-8531-2014; Kolomensky, Yury/I-3510-2015; Pattavina, Luca/I-7498-2015; Maruyama, Reina/A-1064-2013; Pallavicini, Marco/G-5500-2012 OI Clemenza, Massimiliano/0000-0002-8064-8936; Gotti, Claudio/0000-0003-2501-9608; Pessina, Gianluigi Ezio/0000-0003-3700-9757; Goett, Johnny/0000-0002-3685-2227; ARDITO, RAFFAELE/0000-0002-4271-9190; Bersani, Andrea/0000-0003-3276-5713; Faccini, Riccardo/0000-0003-2613-5141; Ligi, Carlo/0000-0001-7943-7704; Gironi, Luca/0000-0003-2019-0967; capelli, silvia/0000-0002-0300-2752; Ma, Yu-Gang/0000-0002-0233-9900; Casali, Nicola/0000-0003-3669-8247; Han, Ke/0000-0002-1609-7367; Keppel, Giorgio/0000-0003-4579-3342; azzolini, oscar/0000-0003-3951-0537; Gutierrez, Thomas/0000-0002-0330-6414; Canonica, Lucia/0000-0001-8734-206X; Vignati, Marco/0000-0002-8945-1128; Giachero, Andrea/0000-0003-0493-695X; Bellini, Fabio/0000-0002-2936-660X; Sangiorgio, Samuele/0000-0002-4792-7802; Nucciotti, Angelo/0000-0002-8458-1556; Martinez, Maria/0000-0002-9043-4691; Di Domizio, Sergio/0000-0003-2863-5895; Ferri, Elena/0000-0003-1425-3669; Kolomensky, Yury/0000-0001-8496-9975; Pattavina, Luca/0000-0003-4192-849X; Maruyama, Reina/0000-0003-2794-512X; Pallavicini, Marco/0000-0001-7309-3023 FU Istituto Nazionale di Fisica Nucleare (INFN); Office of Science, of the U.S. Department of Energy [DE-AC02-05CH11231 and DE-AC52-07NA27344]; DOE Office of Nuclear Physics [DE-FG02-0SER41551, DEFG0300ER41138]; National Science Foundation [NSF-PHY-0605119, NSFIY-0500337, NSF-NW-0855311, NSF-11 IY-0902171]; Alfred P. Sloan Foundation; University of Wisconsin Foundation FX The CUORE Collaboration thanks the Directors and Staff of the Laboratori Nazionali del Gran Sasso and the technical staffs of our Laboratories. This work was supported by the Istituto Nazionale di Fisica Nucleare (INFN); the Director, Office of Science, of the U.S. Department of Energy under Contract Nos. DE-AC02-05CH11231 and DE-AC52-07NA27344; t he DOE Office of Nuclear Physics under Contract Nos. DE-FG02-0SER41551 and DEFG0300ER41138: the National Science Foundation under Grant Nos. NSF-PHY-0605119. NSFIY-0500337, NSF-NW-0855311, and NSF-11 IY-0902171; the Alfred P. Sloan Foundation; and the University of Wisconsin Foundation. NR 40 TC 7 Z9 7 U1 3 U2 35 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1475-7516 J9 J COSMOL ASTROPART P JI J. Cosmol. Astropart. Phys. PD JAN PY 2013 IS 1 AR 038 DI 10.1088/1475-7516/2013/01/038 PG 16 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 086EE UT WOS:000314665600038 ER PT J AU Cheng, HC Huang, WC Low, I Shaughnessy, G AF Cheng, Hsin-Chia Huang, Wei-Chih Low, Ian Shaughnessy, Gabe TI The case for three-body decaying dark matter SO JOURNAL OF COSMOLOGY AND ASTROPARTICLE PHYSICS LA English DT Article DE dark matter theory; CMBR experiments; cosmic ray theory; supersymmetry and cosmology ID COSMIC-RAYS; FERMI; CONSTRAINTS; PAMELA AB Fermi-LAT has confirmed the excess in cosmic positron fraction observed by PAMELA, which could be explained by dark matter annihilating or decaying in the center of the galaxy. Most existing models postulate that the dark matter annihilates or decays into final states with two or four leptons, which would produce diffuse gamma ray emissions that are in tension with data measured by Fermi-LAT. We point out that the tension could be alleviated if the dark matter decays into three-body final states with a pair of leptons and a missing particle. Using the goldstino decay in a certain class of supersymmetric theories as a prime example, we demonstrate that simultaneous fits to the total e(+) + e(-) and the fractional e(+)/e(-) fluxes from Fermi-LAT and PAMELA could be achieved for a 2 TeV parent particle and a 1 TeV missing particle, without being constrained by gamma-ray measurements. By studying different effective operators giving rise to the dark matter decay, we show that this feature is generic for three-body decaying dark matter containing a missing particle. Constraints on the hadronic decay widths from the cosmic anti-proton spectra are also discussed. C1 [Cheng, Hsin-Chia] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. [Huang, Wei-Chih] SISSA, I-34136 Trieste, Italy. [Huang, Wei-Chih] Ist Nazl Fis Nucl, Sez Trieste, I-34136 Trieste, Italy. [Low, Ian; Shaughnessy, Gabe] Argonne Natl Lab, High Energy Phys Div, Argonne, IL 60439 USA. [Low, Ian; Shaughnessy, Gabe] Northwestern Univ, Dept Phys & Astron, Evanston, IL 60208 USA. [Shaughnessy, Gabe] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. RP Cheng, HC (reprint author), Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. EM cheng@physics.ucdavis.edu; whuang@sissa.it; ilow@northwestern.edu; shaughnessy@wisc.edu FU U.S. Department of Energy [DE-AC02-06CH11357, DE-FG02-91ER40684, DE-FG02-95ER40896] FX This work was supported in part by the U.S. Department of Energy under contracts No. DE-AC02-06CH11357, No. DE-FG02-91ER40684 and No. DE-FG02-95ER40896. We thank Marco Cirelli for pointing out the Fermi-LAT EGB data, useful discussions on diffuse gamma rays and help with MATHEMATICA (R) codes in [40]. H.-C.C. would like to thank the hospitality of Fermi lab Theory Group and Academia Sinica in Taiwan, and W.-C.H. would like to thank the hospitality of Physics Division of National Center for Theoretical Sciences (NCTS) in Taiwan, where part of this work was performed. NR 67 TC 3 Z9 3 U1 0 U2 5 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1475-7516 J9 J COSMOL ASTROPART P JI J. Cosmol. Astropart. Phys. PD JAN PY 2013 IS 1 AR 033 DI 10.1088/1475-7516/2013/01/033 PG 28 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 086EE UT WOS:000314665600033 ER PT J AU Lin, GY Cosimbescu, L Karin, NJ Gutowska, A Tarasevich, BJ AF Lin, Genyao Cosimbescu, Lelia Karin, Norman J. Gutowska, Anna Tarasevich, Barbara J. TI Injectable and thermogelling hydrogels of PCL-g-PEG: mechanisms, rheological and enzymatic degradation properties SO JOURNAL OF MATERIALS CHEMISTRY B LA English DT Article ID COPOLYMER AQUEOUS-SOLUTIONS; DRUG-DELIVERY; BIOMEDICAL APPLICATIONS; POLY(ETHYLENE GLYCOL); EPSILON-CAPROLACTONE; TRIBLOCK COPOLYMERS; RESPONSIVE POLYMERS; DIBLOCK COPOLYMERS; BLOCK-COPOLYMERS; MICHAEL ADDITION AB We report new injectable and thermosensitive hydrogels from polycaprolactone-graft-polyethylene glycol (PCL-g-PEG). The PCL-g-PEG polymer aqueous solution was injectable and formed a physical hydrogel at human body temperature. The rheological properties, sol-gel transition mechanisms, and in vitro degradation properties of PCL-g-PEG hydrogels were investigated. Rheological results demonstrate that hydrogels with tunable storage moduli (G') that span four orders of magnitude, from 0.2 to 5500 Pa, can be obtained by varying polymer concentrations. Hydrophobic dye solubilization, dynamic light scattering, and X-ray diffraction results suggest that micelle aggregation and partial crystallization of the polycaprolactone segment lead to the sol-gel transition with increasing temperature. The degradation of PCL-g-PEG hydrogels was slow in the absence of the enzyme lipase, but can be substantially increased by lipase in a concentration-dependent manner. The PCL-g-PEG hydrogel has a low critical gelation concentration, high storage modulus, and easily handled solid morphology, representing great advantages over our previously developed structurally analogous PLGA-g-PEG. The results presented showcase the potential biomedical application of the versatile PCL-g-PEG hydrogels. C1 [Lin, Genyao; Cosimbescu, Lelia; Karin, Norman J.; Tarasevich, Barbara J.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Gutowska, Anna] Adv Imaging Technol, Richland, WA 99352 USA. RP Lin, GY (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM Genyao.Lin@pnnl.gov; Barbara.Tarasevich@pnnl.gov RI Lin, Genyao /G-1062-2011 FU Battelle Pacific Northwest Division's Independent Research and Development Program; Washington State Life Sciences Discovery Fund FX This project was supported by Battelle Pacific Northwest Division's Independent Research and Development Program and the Washington State Life Sciences Discovery Fund. NR 63 TC 17 Z9 17 U1 3 U2 74 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2050-750X J9 J MATER CHEM B JI J. Mat. Chem. B PY 2013 VL 1 IS 9 BP 1249 EP 1255 DI 10.1039/c2tb00468b PG 7 WC Materials Science, Biomaterials SC Materials Science GA 087YY UT WOS:000314801900007 ER PT J AU Shao, M Yan, L Li, MX Ilia, I Hu, B AF Shao, Ming Yan, Liang Li, Mingxing Ilia, Ivanov Hu, Bin TI Triplet-charge annihilation versus triplet-triplet annihilation in organic semiconductors SO JOURNAL OF MATERIALS CHEMISTRY C LA English DT Article ID LIGHT-EMITTING DEVICES; MAGNETIC-FIELD; ELECTROPHOSPHORESCENT DEVICES; ELECTROLUMINESCENT DEVICES; MUTUAL ANNIHILATION; CONJUGATED POLYMERS; ENERGY-TRANSFER; ANTHRACENE; EMISSION; CRYSTALS AB A triplet can annihilate with a charge or a triplet, generating triplet-charge annihilation (TCA) or triplet-triplet annihilation (TTA) in organic semiconductors. On one hand, the TCA and TTA are critical issues to improve optoelectronic responses by using triplet states. On the other hand, the TCA and TTA are important spin-dependent processes to generate magneto-optoelectronic responses. Our experimental studies find that the TCA is a dominant process over TTA in organic semiconductors. Specifically, we separately confine triplets with charges or with triplets towards the generation of TCA and TTA by adjusting triplet density, charge confinement, and charge/exciton ratio based on organic light-emitting diodes. We then use magnetic field effects of electroluminescence (MFEEL) as an experimental tool to study the generation of TCA and TTA. We observe that the electroluminescence can show a negative response to an applied magnetic field, generating a negative MFEEL, when triplets and charges are simultaneously confined within close proximity by using interfacial confinement with unbalanced charge/exciton ratio. In contrast, the electroluminescence only exhibits a positive MFEEL when triplets are confined within close proximity by using interfacial confinement without unbalanced charge/exciton ratio. Therefore, it can be concluded from our MFEEL results that the TCA is a dominant process to annihilate triplets over TTA. Clearly, this experimental finding provides a new understanding on controlling triplets-related optoelectronic and magneto-optoelectronic processes in organic semiconductors. C1 [Shao, Ming; Yan, Liang; Li, Mingxing; Hu, Bin] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Ilia, Ivanov] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Hu, Bin] Huazhong Univ Sci & Technol, Wu Han Natl Lab Optoelect, Wuhan 430074, Peoples R China. RP Shao, M (reprint author), Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. EM bhu@utk.edu RI Hu, Bin/A-2954-2015; Yan, Liang/H-6471-2011 OI Hu, Bin/0000-0002-1573-7625; Yan, Liang/0000-0003-4122-7466 FU Air Force Office of Scientific Research (AFOSR) [FA9550-11-1-0082]; NSF [ECCS-0644945, ECCS-1102011]; Oak Ridge National Laboratory by the Division of Scientific User Facilities, U.S. Department of Energy; International Cooperation and Exchange Program at the National Natural Science Foundation of China [21161160445]; Photovoltaic Project [61077020]; National Natural Science Foundation of China; National Significant Program of China [2013CB922104]; Center for Nanophase Materials Sciences [CNMS2012-106, CNMS2012-107] FX The authors would like to acknowledge the financial supports from Air Force Office of Scientific Research (AFOSR) under the grant number FA9550-11-1-0082 and from NSF under grant numbers ECCS-0644945 and ECCS-1102011. This research was partially conducted at the Center for Nanophase Materials Sciences based on user project (CNMS2012-106 and CNMS2012-107), which is sponsored at Oak Ridge National Laboratory by the Division of Scientific User Facilities, U.S. Department of Energy. We also acknowledge the support from International Cooperation and Exchange Program (grant no. 21161160445) at the National Natural Science Foundation of China. This work was also supported by the Photovoltaic Project (grant no. 61077020) funded by the National Natural Science Foundation of China. The funding support from National Significant Program (Quantum Control: 2013CB922104) of China is also acknowledged. NR 50 TC 20 Z9 24 U1 6 U2 66 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2050-7526 EI 2050-7534 J9 J MATER CHEM C JI J. Mater. Chem. C PY 2013 VL 1 IS 7 BP 1330 EP 1336 DI 10.1039/c2tc00329e PG 7 WC Materials Science, Multidisciplinary; Physics, Applied SC Materials Science; Physics GA 088AW UT WOS:000314807200006 ER PT J AU Johnson, RS Wheeler, DR Dirk, SM AF Johnson, Ross S. Wheeler, David R. Dirk, Shawn M. TI Photolithographic patterning of alkoxy substituted poly(p-phenylenevinylene)s from xanthate precursors SO JOURNAL OF MATERIALS CHEMISTRY C LA English DT Article ID FIELD-EFFECT TRANSISTORS; CONJUGATED POLYMERS; DEVICES; PERFORMANCE; VINYLENE); LITHOGRAPHY; RESOLUTION; SURFACES; CONTACT; FILMS AB Conducting polymers are seeing ever-increased use in electronic and optoelectronic applications. While a variety of techniques are available to pattern conducting polymers, the demand for low cost, high throughput, and good spatial resolution continues to drive research efforts in this area. We have previously developed a method to pattern poly(p-phenylenevinylene) (PPV) using contact photolithography. Here, the synthesis, characterization, and photopatterning of alkoxy substituted PPVs (a much more commonly utilized derivative) is presented. Utilizing a photoacid generator, the polymer systems are demonstrated to pattern to one micron spatial resolution. The patterning process is demonstrated to have little effect on the polymers properties as the materials retain good optical characteristics and high conductivities upon doping. C1 [Johnson, Ross S.; Dirk, Shawn M.] Sandia Natl Labs, Organ Mat Dept, Albuquerque, NM 87185 USA. [Wheeler, David R.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Johnson, RS (reprint author), DuPont Expt Stn, 200 Powder Mill Rd, Wilmington, DE 19880 USA. EM ross.s.johnson@dupont.com FU Laboratory Directed Research and Development program at Sandia National Laboratories; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; Lockheed Martin Corporation FX The Authors thank Patrick Finnegan for assistance with obtaining optical and fluorescence images as well as profilometry measurements. This work was supported by the Laboratory Directed Research and Development program at Sandia National Laboratories. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 50 TC 2 Z9 2 U1 0 U2 22 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2050-7526 EI 2050-7534 J9 J MATER CHEM C JI J. Mater. Chem. C PY 2013 VL 1 IS 7 BP 1428 EP 1433 DI 10.1039/c2tc00599a PG 6 WC Materials Science, Multidisciplinary; Physics, Applied SC Materials Science; Physics GA 088AW UT WOS:000314807200019 ER PT J AU Wang, XJ Xiao, HY Zu, XT Zhang, Y Weber, WJ AF Wang, X. J. Xiao, H. Y. Zu, X. T. Zhang, Y. Weber, W. J. TI Ab initio molecular dynamics simulations of ion-solid interactions in Gd2Zr2O7 and Gd2Ti2O7 SO JOURNAL OF MATERIALS CHEMISTRY C LA English DT Article ID RADIATION TOLERANCE; OXIDE PYROCHLORES; NUCLEAR-WASTE; DISPLACEMENT; IRRADIATION; IMMOBILIZATION; PLUTONIUM; FLUORITE; PSEUDOPOTENTIALS; AMORPHIZATION AB The development of the ab initio molecular dynamics (AIMD) method has made it a powerful tool in describing ion-solid interactions in materials, with the determination of threshold displacement energies with ab initio accuracy, and prediction of a new mechanism for defect generation and new defective states that are different from classical molecular dynamics (MD) simulations. In the present work, this method is employed to study the low energy recoil events in Gd2Zr2O7 and Gd2Ti2O7. The weighted average threshold displacement energies in Gd2Zr2O7 are determined to be 38.8 eV for Gd, 41.4 eV for Zr, 18.6 eV for O-48f, and 15.6 eV for O-8b, which are smaller than the respective values of 41.8, >53.8, 22.6 and 16.2 eV in Gd2Ti2O7. It reveals that all the ions in Gd2Zr2O7 are more easily displaced than those in Gd2Ti2O7, and anion order-disorder is more likely to be involved in the displacement events than cation disordering. The average charge transfer from the primary knock-on atom to its neighbors is estimated to be similar to 0.15, similar to 0.11 to 0.27 and similar to 0.1 to 0.13 vertical bar e vertical bar for Gd, Zr (or Ti), and O, respectively. Neglecting the charge transfer in the interatomic potentials may result in the larger threshold displacement energies in classical MD. C1 [Wang, X. J.; Zu, X. T.] Univ Elect Sci & Technol China, Sch Phys Elect, Chengdu 610054, Peoples R China. [Xiao, H. Y.; Zhang, Y.; Weber, W. J.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Zhang, Y.; Weber, W. J.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Wang, XJ (reprint author), Univ Elect Sci & Technol China, Sch Phys Elect, Chengdu 610054, Peoples R China. EM hxiao@utk.edu RI Weber, William/A-4177-2008; wang, xiangjian/K-4923-2012 OI Weber, William/0000-0002-9017-7365; FU National Natural Science Foundation of China [11004023]; Scientific Research Foundation for the Returned Overseas Chinese Scholars, State Education Ministry; U.S. Department of Energy, Office of Science, Basic Energy Science, Materials Sciences and Engineering Division FX X.J. Wang was supported by the National Natural Science Foundation of China (Grant no. 11004023) and by the Project Sponsored by the Scientific Research Foundation for the Returned Overseas Chinese Scholars, State Education Ministry. W.J. Weber, Y. Zhang and H.Y. Xiao were supported by the U.S. Department of Energy, Office of Science, Basic Energy Science, Materials Sciences and Engineering Division. The theoretical calculations were partially performed using the supercomputer resources at the Environmental Molecular Sciences Laboratory (EMSL) located at the Pacific Northwest National Laboratory. NR 43 TC 8 Z9 8 U1 3 U2 55 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2050-7526 J9 J MATER CHEM C JI J. Mater. Chem. C PY 2013 VL 1 IS 8 BP 1665 EP 1673 DI 10.1039/c2tc00192f PG 9 WC Materials Science, Multidisciplinary; Physics, Applied SC Materials Science; Physics GA 088BC UT WOS:000314807800018 ER PT J AU zur Borg, L Lee, D Lim, J Bae, WK Park, M Lee, S Lee, C Char, K Zentel, R AF zur Borg, Lisa Lee, Donggu Lim, Jaehoon Bae, Wan Ki Park, Myeongjin Lee, Seonghoon Lee, Changhee Char, Kookheon Zentel, Rudolf TI The effect of band gap alignment on the hole transport from semiconducting block copolymers to quantum dots SO JOURNAL OF MATERIALS CHEMISTRY C LA English DT Article ID LIGHT-EMITTING-DIODES; LIVING RADICAL POLYMERIZATION; OPTICAL-PROPERTIES; RAFT PROCESS; ENERGY-LEVELS; NANOCRYSTALS; POLYMERS; DEVICES; UPDATE AB Semiconducting hole transporting block copolymers were chemically modified to adjust their energy levels to that of CdSe/CdS/CdZnS red quantum dots. Hybrids with optimized energy levels could be used to build strongly improved quantum dot based LEDs (QLEDs). C1 [zur Borg, Lisa; Zentel, Rudolf] Johannes Gutenberg Univ Mainz, Inst Organ Chem, D-55128 Mainz, Germany. [Lee, Donggu; Park, Myeongjin; Lee, Changhee] Seoul Natl Univ, Interuniv Semicond Res Ctr, Dept Elect & Comp Engn, Seoul 151744, South Korea. [Lim, Jaehoon; Char, Kookheon] Seoul Natl Univ, WCU Program Chem Convergence Energy & Environm, Natl Creat Res Initiat Ctr Intelligent Hybrids, Sch Chem & Biol Engn, Seoul 151744, South Korea. [Bae, Wan Ki] Los Alamos Natl Lab, Div Chem, Los Alamos, NM 87545 USA. [Lee, Seonghoon] Seoul Natl Univ, Sch Chem, Seoul 151747, South Korea. RP zur Borg, L (reprint author), Johannes Gutenberg Univ Mainz, Inst Organ Chem, Duesbergweg 10-14, D-55128 Mainz, Germany. EM shnlee@snu.ac.kr; chlee7@snu.ac.kr; khchar@plaza.snu.ac.kr; zentel@uni-mainz.de RI Lee, Changhee/A-2471-2009; Zentel, Rudolf/D-4542-2011 OI Lee, Changhee/0000-0003-2800-8250; FU International Research Training Group (IRTG): Self Organized Materials for Optoelectronics [GRK 1404]; National Research Foundation of Korea (NRF) through the Acceleration Research Program [R0A-2008-000-20108-0]; National Creative Research Initiative Center for Intelligent Hybrids [2010-0018290]; WCU C2E2 [R31-10013]; BK21 Program; Leading Foreign Research Institute Recruitment Program [2011-0030065]; [NRF-2009-C1AAA001-2009-0093282] FX This work was financially supported by the International Research Training Group (IRTG): Self Organized Materials for Optoelectronics (GRK 1404). It was also supported by the National Research Foundation of Korea (NRF) through the Acceleration Research Program (R0A-2008-000-20108-0), the grant (NRF-2009-C1AAA001-2009-0093282), the National Creative Research Initiative Center for Intelligent Hybrids (no. 2010-0018290), WCU C2E2 (R31-10013) and the BK21 Program. This work was also partly supported by Leading Foreign Research Institute Recruitment Program (2011-0030065). NR 32 TC 9 Z9 9 U1 1 U2 63 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2050-7526 J9 J MATER CHEM C JI J. Mater. Chem. C PY 2013 VL 1 IS 9 BP 1722 EP 1726 DI 10.1039/c3tc00837a PG 5 WC Materials Science, Multidisciplinary; Physics, Applied SC Materials Science; Physics GA 088BP UT WOS:000314809100005 ER PT J AU Rainbolt, JE Koech, PK Polikarpov, E Swensen, JS Cosimbescu, L Von Ruden, A Wang, L Sapochak, LS Padmaperuma, AB Gaspar, DJ AF Rainbolt, James E. Koech, Phillip K. Polikarpov, Evgueni Swensen, James S. Cosimbescu, Lelia Von Ruden, Amber Wang, Liang Sapochak, Linda S. Padmaperuma, Asanga B. Gaspar, Daniel J. TI Synthesis and characterization of p-type conductivity dopant 2-(3-(adamantan-1-yl)propyl)-3,5,6-trifluoro-7,7,8,8-tetracyanoquinodime thane SO JOURNAL OF MATERIALS CHEMISTRY C LA English DT Article ID ORGANIC ELECTROLUMINESCENT DEVICES; CORRELATED MOLECULAR CALCULATIONS; MOLYBDENUM DITHIOLENE COMPLEX; LIGHT-EMITTING DEVICES; GAUSSIAN-BASIS SETS; ELECTRICAL-PROPERTIES; TRANSPORT; PHTHALOCYANINE; SEMICONDUCTORS; FILMS AB We report the synthesis and characterization of 2-(3-(adamantan-1-yl)propyl)-3,5,6-trifluoro-7,7,8,8-tetracyanoquinodimethane (F3TCNQ-Ad1), a substituted analog of 2,3,5,6-tetrafluoro-7,7,8,8-tetracyanoquinodimethane (F4TCNQ), designed for p-type conductivity doping. The dopant is designed as a model for substituted alternatives to F4TCNQ that maintain similar electronic properties with the goal of engineering dopants with superior fabrication characteristics over F4TCNQ. We describe the design strategy for F3TCNQ-Ad1 based on molecular modeling predictions that substitution of a single fluorine atom of F4TCNQ has little effect on the electronic properties of the molecule. Photophysical and electrochemical characterization reveal that the adamantyl substituent in F3TCNQ-Ad1 does not significantly alter the electronic properties of the substituted dopant relative to F4TCNQ. Unfortunately, F3TCNQ-Ad1 degrades under standard sublimation conditions, preventing sublimation deposition processing. Instead, hole-only devices were made via solution-processing of the p-doped films with the structure glass/ITO/2.3 x 10(3) angstrom PVK:(MTDATA:dopant)/2.0 x 10(2) angstrom Au/1.0 x 10(3) angstrom Al, where dopant is either F4TCNQ or F3TCNQ-Ad1. We demonstrate that F3TCNQ-Ad1 increased the conductivity of the films by at least 1000 times compared to an undoped device. C1 [Rainbolt, James E.; Koech, Phillip K.; Polikarpov, Evgueni; Swensen, James S.; Cosimbescu, Lelia; Von Ruden, Amber; Wang, Liang; Padmaperuma, Asanga B.; Gaspar, Daniel J.] Pacific NW Natl Lab, Energy & Environm Directorate, Appl Mat Sci Grp, Richland, WA 99352 USA. [Sapochak, Linda S.] Natl Sci Fdn, Math & Phys Sci Directorate, Div Mat Res, Arlington, VA 22230 USA. RP Rainbolt, JE (reprint author), Pacific NW Natl Lab, Energy & Environm Directorate, Appl Mat Sci Grp, 902 Battelle Blvd,POB 999,MSIN K2-44, Richland, WA 99352 USA. EM phillip.koech@pnnl.gov RI Gaspar, Dan/H-6166-2011; OI Gaspar, Daniel/0000-0002-8089-810X; Koech, Phillip/0000-0003-2996-0593 FU U. S. Dept. of Energy [M6743231, M68004043]; U.S. Department of Energy (DOE) [DE-AC06-76RLO 1830] FX The authors would like to thank Dr Zihua Zhu (PNNL) for performing time-of-flight secondary ion mass spectrometry analysis (ToF-SIMS). This work was funded by the Solid Sate Lighting Program of the U. S. Dept. of Energy, within the Building Technologies Program (BT), (Award nos M6743231 and M68004043) and managed by the National Energy Technology Laboratory (NETL). A portion of this research was performed using Environmental Molecular Sciences Laboratory (EMSL). Computations were carried out using "NWChem, A Computational Chemistry Package for Parallel Computers, Version 5.1" (2007), and Extensible Computational Chemistry Environment (ECCE), A Problem Solving Environment for Computational Chemistry, So. ware Version 6.0" (2009), as developed and distributed by Pacific Northwest National Laboratory, and funded by the U.S. Department of Energy. Pacific Northwest National Laboratory is operated by Battelle Memorial Institute for the U.S. Department of Energy (DOE) under Contract no. DE-AC06-76RLO 1830. NR 37 TC 7 Z9 7 U1 7 U2 48 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2050-7526 J9 J MATER CHEM C JI J. Mater. Chem. C PY 2013 VL 1 IS 9 BP 1876 EP 1884 DI 10.1039/c3tc00068k PG 9 WC Materials Science, Multidisciplinary; Physics, Applied SC Materials Science; Physics GA 088BP UT WOS:000314809100025 ER PT J AU Cai, W Chen, Q Cherepy, N Dooraghi, A Kishpaugh, D Chatziioannou, A Payne, S Xiang, WD Pei, QB AF Cai, Wen Chen, Qi Cherepy, Nerine Dooraghi, Alex Kishpaugh, David Chatziioannou, Arion Payne, Stephen Xiang, Weidong Pei, Qibing TI Synthesis of bulk-size transparent gadolinium oxide-polymer nanocomposites for gamma ray spectroscopy SO JOURNAL OF MATERIALS CHEMISTRY C LA English DT Article ID LOADED PLASTIC SCINTILLATORS; EXCITATION-ENERGY TRANSFER; RADIATION DETECTION; OPTICAL-PROPERTIES; ORGANOMETALLICS; NANOCRYSTALS; COMPOSITES; DISPERSION; TRIPHENYLBISMUTH; NANOPARTICLES AB Heavy element loaded polymer composites have long been proposed to detect high energy X- and gamma-rays upon scintillation. The previously reported bulk composite scintillators have achieved limited success because of the diminished light output resulting from fluorescence quenching and opacity. We demonstrate the synthesis of a transparent nanocomposite comprising gadolinium oxide nanocrystals uniformly dispersed in bulk-size samples at a high loading content. The strategy to avoid luminescence quenching and opacity in the nanocomposite was successfully deployed, which led to the radioluminescence light yield of up to 27 000/MeV, about twice as much as standard commercial plastic scintillators. Nanocomposites monoliths (14 mm diameter by 3 mm thickness) with 31 wt% loading of nanocrystals generated a photoelectric peak for Cs-137 gamma (662 keV) with 11.4% energy resolution. C1 [Cai, Wen; Chen, Qi; Kishpaugh, David; Pei, Qibing] Univ Calif Los Angeles, Dept Mat Sci & Engn, Los Angeles, CA 90095 USA. [Cherepy, Nerine; Payne, Stephen] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Dooraghi, Alex; Chatziioannou, Arion] Univ Calif Los Angeles, Dept Mol & Med Pharmacol, Los Angeles, CA 90095 USA. [Cai, Wen; Xiang, Weidong] Tongji Univ, Sch Mat Sci & Engn, Shanghai 201804, Peoples R China. RP Cai, W (reprint author), Univ Calif Los Angeles, Dept Mat Sci & Engn, Los Angeles, CA 90095 USA. EM qpei@seas.ucla.edu RI Cherepy, Nerine/F-6176-2013; Pei, Qibing/N-7497-2015 OI Cherepy, Nerine/0000-0001-8561-923X; FU Defense Threat Reduction Agency of the United States Department of Defense [HDTRA1-07-1-0028]; China Scholarship Council; U.S. DOE, NNSA, Office of Defense Nuclear Nonproliferation, Office of Nonproliferation Research and Development [NA-22] FX This work was supported by the Defense Threat Reduction Agency of the United States Department of Defense, Contract # HDTRA1-07-1-0028. W.C. acknowledges the financial support of the China Scholarship Council. The LLNL contribution is funded by the U.S. DOE, NNSA, Office of Defense Nuclear Nonproliferation, Office of Nonproliferation Research and Development (NA-22). NR 45 TC 21 Z9 21 U1 7 U2 47 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2050-7526 J9 J MATER CHEM C JI J. Mater. Chem. C PY 2013 VL 1 IS 10 BP 1970 EP 1976 DI 10.1039/c2tc00245k PG 7 WC Materials Science, Multidisciplinary; Physics, Applied SC Materials Science; Physics GA 089FA UT WOS:000314894300007 PM 26478816 ER PT J AU Woo, H Lim, J Lee, Y Sung, J Shin, H Oh, JM Choi, M Yoon, H Bae, WK Char, K AF Woo, Heeje Lim, Jaehoon Lee, Yeonju Sung, Jinwoo Shin, Hyunkwon Oh, Jin Mok Choi, Moongoo Yoon, Hyunsik Bae, Wan Ki Char, Kookheon TI Robust, processable, and bright quantum dot/organosilicate hybrid films with uniform QD distribution based on thiol-containing organosilicate ligands SO JOURNAL OF MATERIALS CHEMISTRY C LA English DT Article ID LIGHT-EMITTING-DIODES; SEMICONDUCTOR NANOCRYSTALS; SOLAR-CELLS; DOTS; CLUSTERS; POLYMER; SILSESQUIOXANES; DEVICES; WELL AB Robust, processable, and bright quantum dot/organosilicate (QD/OS) hybrid films with uniform QD distribution are successfully demonstrated by grafting thiol-containing polymeric organosilicate (OS) ligands to the surface of QDs. It is found that the surface modified QDs show almost the same optical properties (i.e., in terms of emission PL spectra and quantum yields (QYs)) as those of pristine QDs initially covered with oleic acids. The QD/OS hybrid films based on the surface modified QDs show the uniform distribution of QDs within the films with all the beneficial properties such as high QY, improved environmental resistance against hydrochloric acid, and excellent optical transparency in the visible range. In addition, red, green, blue, and white QD/OS hybrid films with high color purity and a down-conversion film, based on a mixture of red and green QDs, placed on top of a blue LED chip showing white emission were also successfully demonstrated with the QD/OS hybrids. We further demonstrate that cylinder-patterned QD/OS hybrid films are possible simply by applying unconventional imprint lithography. The QD/OS hybrid films with uniform distribution of QDs within the films could thus be applied as practical platforms, which have easy processability, high QY, and environmental stability, for optical devices based on functional nanocrystals. C1 [Woo, Heeje; Lim, Jaehoon; Lee, Yeonju; Char, Kookheon] Seoul Natl Univ, Natl Creat Res Initiat Ctr Intelligent Hybrids, WCU Program Chem Convergence Energy & Environm, Sch Chem & Biol Engn, Seoul 151744, South Korea. [Sung, Jinwoo; Shin, Hyunkwon; Oh, Jin Mok; Choi, Moongoo] LG Elect, LGE Adv Res Inst, Mat & Devices Lab, Seoul 137724, South Korea. [Yoon, Hyunsik] Seoul Natl Univ Sci & Technol, Dept Chem Engn, Seoul 139743, South Korea. [Bae, Wan Ki] Los Alamos Natl Lab, Div Chem, Los Alamos, NM 87544 USA. RP Woo, H (reprint author), Seoul Natl Univ, Natl Creat Res Initiat Ctr Intelligent Hybrids, WCU Program Chem Convergence Energy & Environm, Sch Chem & Biol Engn, 1 Gwanak Ro, Seoul 151744, South Korea. EM khchar@plaza.snu.ac.kr FU National Research Foundation of Korea (NRF); Korean Ministry of Education, Science and Technology (MEST) through The National Creative Research Initiative Program for "Intelligent Hybrids Research Center" [2010-0018290]; WCU Program of Chemical Convergence for Energy and Environment [R31-10013]; Leading Foreign Research Institute Recruitment Program [2011-0030065]; Brain Korea 21 Program in Chemical Engineering of Seoul National University FX This work was financially supported by the National Research Foundation of Korea (NRF) funded by the Korean Ministry of Education, Science and Technology (MEST) through The National Creative Research Initiative Program for "Intelligent Hybrids Research Center" (no. 2010-0018290), the WCU Program of Chemical Convergence for Energy and Environment (R31-10013), Leading Foreign Research Institute Recruitment Program (2011-0030065), and the Brain Korea 21 Program in Chemical Engineering of Seoul National University. This work was also partially supported by the financial support from LG Electronics. NR 35 TC 9 Z9 10 U1 3 U2 37 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2050-7526 J9 J MATER CHEM C JI J. Mater. Chem. C PY 2013 VL 1 IS 10 BP 1983 EP 1989 DI 10.1039/c3tc00719g PG 7 WC Materials Science, Multidisciplinary; Physics, Applied SC Materials Science; Physics GA 089FA UT WOS:000314894300009 ER PT J AU Ramanathan, M Tseng, YC Ariga, K Darling, SB AF Ramanathan, Muruganathan Tseng, Yu-Chih Ariga, Katsuhiko Darling, Seth B. TI Emerging trends in metal-containing block copolymers: synthesis, self-assembly, and nanomanufacturing applications SO JOURNAL OF MATERIALS CHEMISTRY C LA English DT Article ID ATOMIC LAYER DEPOSITION; SEQUENTIAL INFILTRATION SYNTHESIS; ORGANOMETALLIC POLYMER CHEMISTRY; LIVING RADICAL POLYMERIZATION; ABC TRIBLOCK TERPOLYMER; ORDERED SQUARE ARRAYS; THIN-FILMS; POLYFERROCENE-BLOCK; DIBLOCK COPOLYMERS; MAIN-CHAIN AB Block copolymers with metals confined in one or more blocks are emerging as candidate materials for nanomanufacturing applications due to their unprecedented nanoscale pattern transfer capabilities. In this article we highlight recent developments in metal-containing block copolymers in terms of their novel synthetic methodologies with particular emphasis on sequential infiltration synthesis, their hierarchical self-assembly from nano, meso, and submicron scales, and their applications as an etch mask for high-throughput, high-aspect-ratio nano and meso scale patterning. C1 [Ramanathan, Muruganathan] Oak Ridge Natl Lab, CNMS, Oak Ridge, TN 37830 USA. [Tseng, Yu-Chih] Nat Resources Canada, CanmetMATERIALS, Hamilton, ON L8P 0A5, Canada. [Tseng, Yu-Chih] McMaster Univ, Dept Mech Engn, Hamilton, ON L8S 4L7, Canada. [Ariga, Katsuhiko] NIMS, WPI Res Ctr Mat Nanoarchitecton MANA, Tsukuba, Ibaraki 3050044, Japan. [Darling, Seth B.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Darling, Seth B.] Univ Chicago, Inst Mol Engn, Chicago, IL 60637 USA. RP Ramanathan, M (reprint author), Oak Ridge Natl Lab, CNMS, Oak Ridge, TN 37830 USA. EM nmr@ornl.gov RI ARIGA, Katsuhiko/H-2695-2011 FU Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; World Premier International Research Center Initiative (WPI Initiative), MEXT, Japan; Core Research for Evolutional Science and Technology (CREST) program of Japan Science and Technology Agency (JST), Japan; Center for Nanoscale Materials, a U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility [DE-AC02-06CH11357] FX This research was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. This work was also partly supported by World Premier International Research Center Initiative (WPI Initiative), MEXT, Japan and the Core Research for Evolutional Science and Technology (CREST) program of Japan Science and Technology Agency (JST), Japan. This work was performed, in part, at the Center for Nanoscale Materials, a U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility under Contract no. DE-AC02-06CH11357. NR 124 TC 39 Z9 39 U1 3 U2 79 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2050-7526 J9 J MATER CHEM C JI J. Mater. Chem. C PY 2013 VL 1 IS 11 BP 2080 EP 2091 DI 10.1039/c3tc00930k PG 12 WC Materials Science, Multidisciplinary; Physics, Applied SC Materials Science; Physics GA 093CK UT WOS:000315169100001 ER PT J AU Ramanathan, M Lokitz, BS Messman, JM Stafford, CM Kilbey, SM AF Ramanathan, Muruganathan Lokitz, Bradley S. Messman, Jamie M. Stafford, Christopher M. Kilbey, S. Michael, II TI Spontaneous wrinkling in azlactone-based functional polymer thin films in 2D and 3D geometries for guided nanopatterning SO JOURNAL OF MATERIALS CHEMISTRY C LA English DT Article ID FABRICATION; SILICON; MECHANICS; PATTERNS AB We report a simple, one step process for developing wrinkling patterns in azlactone-based polymer thin films and brushes on 2D and 3D surfaces. The polymer used in this work wrinkles spontaneously upon deposition and solidification on a substrate without applying any external strain to the substrate, with the mode of deposition defining the direction of the wrinkles. Wrinkle formation is shown to occur on a variety of substrates over large areas. We also find that a very thin brush-like layer of an azlactone-containing block copolymer also exhibits wrinkled topology. Given the spontaneity and versatility of wrinkle formation, we further demonstrate two proofs-of-concept, (i) that these periodic wrinkled structures are not limited to planar surfaces, but are also developed in complex geometries including tubes, cones and other 3D structures; and (ii) that this one step wrinkling process can be used to guide the deposition of metal nanoparticles and quantum dots, creating a periodic, nanopatterned film. C1 [Ramanathan, Muruganathan; Lokitz, Bradley S.; Messman, Jamie M.; Kilbey, S. Michael, II] Oak Ridge Natl Lab, CNMS, Oak Ridge, TN 37831 USA. [Stafford, Christopher M.] NIST, Mat Sci & Engn Div, Gaithersburg, MD 20899 USA. [Kilbey, S. Michael, II] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. RP Ramanathan, M (reprint author), Oak Ridge Natl Lab, CNMS, Oak Ridge, TN 37831 USA. EM nmr@ornl.gov RI Lokitz, Bradley/Q-2430-2015 OI Lokitz, Bradley/0000-0002-1229-6078 FU Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX This research was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. NR 41 TC 8 Z9 8 U1 0 U2 31 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2050-7526 J9 J MATER CHEM C JI J. Mater. Chem. C PY 2013 VL 1 IS 11 BP 2097 EP 2101 DI 10.1039/c3tc00946g PG 5 WC Materials Science, Multidisciplinary; Physics, Applied SC Materials Science; Physics GA 093CK UT WOS:000315169100003 ER PT J AU Sundaram, SK Sacksteder, CA Weber, TJ Riley, BJ Addleman, RS Harrer, BJ Peterman, JW AF Sundaram, S. K. Sacksteder, Colette A. Weber, Thomas J. Riley, Brian J. Addleman, R. Shane Harrer, Bruce J. Peterman, John W. TI Fourier-transform infrared spectroscopy for rapid screening and live-cell monitoring: application to nanotoxicology SO NANOMEDICINE LA English DT Article DE attenuated total reflectance; cell culture monitoring; Fourier-transform infrared; live-cell monitoring; nanosized particle; nanotoxicology in vitro; rapid screening; spectroscopy; toxicity ID RESEARCH STRATEGIES; SAFETY EVALUATION; NANOSCALE PARTICLES; PROTEIN ADSORPTION; RAMAN-SPECTROSCOPY; FTIR SPECTROSCOPY; NANOMATERIALS; HEALTH; RISK; NANOMEDICINE AB A significant challenge to realize the full potential of nanotechnology for therapeutic and diagnostic applications is to understand and evaluate how live cells interact with an external stimulus, such as a nanosized particle, and the toxicity and broad risk associated with these stimuli. It is difficult to capture the complexity and dynamics of these interactions by following omics-based approaches exclusively, which can be expensive and time-consuming. Attenuated total reflectance-Fourier transform infrared spectroscopy is well suited to provide noninvasive live-cell monitoring of cellular responses to potentially toxic nanosized particles or other stimuli. This alternative approach provides the ability to carry out rapid toxicity screenings and nondisruptive monitoring of live-cell cultures. We review the technical basis of the approach, the instrument configuration and interface with the biological media, the various effects that impact the data, subsequent data analysis and toxicity, and present some preliminary results on live-cell monitoring. C1 [Sundaram, S. K.] Alfred Univ, Kazuo Inamori Sch Engn, Alfred, NY 14802 USA. [Sacksteder, Colette A.; Weber, Thomas J.; Riley, Brian J.; Addleman, R. Shane; Harrer, Bruce J.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Peterman, John W.] Simplex Sci, Middleton, WI 53562 USA. RP Sundaram, SK (reprint author), Alfred Univ, Kazuo Inamori Sch Engn, Alfred, NY 14802 USA. EM sundaram@alfred.edu RI Geracitano, Laura/E-6926-2013; OI Riley, Brian/0000-0002-7745-6730 FU Pacific Northwest National Laboratory, Laboratory Directed Research and Development (LDRD); Technology Maturation Program of the Battelle Memorial Institute; US Department of Energy [DE-AC06-76RLO 1830]; Inamori Professorship at Alfred University by the Kyocera Corporation FX This work was funded by the Pacific Northwest National Laboratory, Laboratory Directed Research and Development (LDRD) as well as by the Technology Maturation Program of the Battelle Memorial Institute. The authors acknowledge the support by C Cejka and E Murphy, J Pounds and J Teeguarden. Pacific Northwest National Laboratory is a multiprogram national laboratory operated by Battelle Memorial Institute for the US Department of Energy under DE-AC06-76RLO 1830. SK Sundaram acknowledges the support of the Inamori Professorship at Alfred University by the Kyocera Corporation. The authors have no other relevant affiliations or financial involvement with any organization or entity with a financial interest in or financial conflict with the subject matter or materials discussed in the manuscript apart from those disclosed. NR 41 TC 2 Z9 2 U1 1 U2 27 PU FUTURE MEDICINE LTD PI LONDON PA UNITEC HOUSE, 3RD FLOOR, 2 ALBERT PLACE, FINCHLEY CENTRAL, LONDON, N3 1QB, ENGLAND SN 1743-5889 J9 NANOMEDICINE-UK JI Nanomedicine PD JAN PY 2013 VL 8 IS 1 BP 145 EP 156 DI 10.2217/NNM.12.186 PG 12 WC Biotechnology & Applied Microbiology; Nanoscience & Nanotechnology SC Biotechnology & Applied Microbiology; Science & Technology - Other Topics GA 084YS UT WOS:000314577800020 PM 23256497 ER PT J AU Crapps, J Clarke, K Katz, J Alexander, DJ Aikin, B Vargas, VD Montalvo, JD Dombrowski, DE Mihaila, B AF Crapps, Justin Clarke, Kester Katz, Joel Alexander, David J. Aikin, Beverly Vargas, Victor D. Montalvo, Joel D. Dombrowski, David E. Mihaila, Bogdan TI Development of the hot isostatic press manufacturing process for monolithic nuclear fuel SO NUCLEAR ENGINEERING AND DESIGN LA English DT Article ID PRACTICAL APPLICATIONS; DIAGRAMS; HIP; DENSIFICATION; CERAMICS; METALS C1 [Crapps, Justin; Clarke, Kester; Katz, Joel; Alexander, David J.; Aikin, Beverly; Vargas, Victor D.; Montalvo, Joel D.; Dombrowski, David E.; Mihaila, Bogdan] Los Alamos Natl Lab, Mat Sci & Technol Div, Los Alamos, NM 87545 USA. RP Mihaila, B (reprint author), Los Alamos Natl Lab, Mat Sci & Technol Div, POB 1663, Los Alamos, NM 87545 USA. EM bmihaila@lanl.gov RI Mihaila, Bogdan/D-8795-2013 OI Mihaila, Bogdan/0000-0002-1489-8814 FU U.S. Department of Energy, Office of the National Nuclear Security Administration, under the Global Threat Reduction Initiative Reactor Convert program FX Work performed in part under the auspices of the U.S. Department of Energy, Office of the National Nuclear Security Administration, under the Global Threat Reduction Initiative Reactor Convert program. NR 25 TC 1 Z9 1 U1 0 U2 9 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0029-5493 J9 NUCL ENG DES JI Nucl. Eng. Des. PD JAN PY 2013 VL 254 BP 43 EP 52 DI 10.1016/j.nucengdes.2012.09.002 PG 10 WC Nuclear Science & Technology SC Nuclear Science & Technology GA 090TF UT WOS:000315002200006 ER PT J AU Lorenzi, S Cammi, A Bortot, S Ponciroli, R Moisseytsev, A AF Lorenzi, S. Cammi, A. Bortot, S. Ponciroli, R. Moisseytsev, A. TI Analytical models for a small LFR core dynamics studies SO NUCLEAR ENGINEERING AND DESIGN LA English DT Article ID FUELS; MOX AB Analytical models for the study of a small Lead-cooled Fast Reactor (LFR) demonstrator (DEMO) core dynamics, in a control-oriented perspective, have been developed aimed at providing a useful, very flexible and straightforward tool allowing relatively quick transient design-basis and stability analyses. A simplified approach has been developed consisting in a lumped-parameter modeling of the coupled neutronics and thermal-hydraulics. The reactor transient responses following both postulated accident initiators such as Unprotected Transient of OverPower (UTOP), Loss of Heat Sink (ULOHS) and Loss of Flow (ULOF), and an emergency SCRAM event have been studied in MATLAB/SIMULINK (R) environment. A benchmark analysis has been then performed by means of the SAS4A/SASSYS-1 Liquid Metal Reactor Code System with the purpose of providing verification for the analytical outcomes of the nonlinear model and indicating how the latter relate to more realistic one-dimensional calculations. As a general result, responses concerning the main core characteristics (namely, power, reactivity, etc.) have turned out to be mutually consistent in terms of both steady-state absolute figures and transient developments, showing discrepancies of the order of only few per cents. DEMO dynamic behavior has been studied through a linear approach as well, so as to enable the use of linear analysis tools allowing to verify the system stability, thanks to the possibility of expressing a physical model in terms of transfer functions or state-space representation. The impact of linearization and point-kinetics one-precursor-group approximation has been further evaluated by examining the respective transient predictions, which have been compared to the nonlinear reference ones for increasing perturbations. An asymptotic stability analysis, according to Lyapunov's definition, is finally presented. (C) 2012 Elsevier B.V. All rights reserved. C1 [Lorenzi, S.; Cammi, A.; Bortot, S.; Ponciroli, R.] Politecn Milan, Nucl Engn Div CeSNEF, Dept Energy, I-20156 Milan, Italy. [Moisseytsev, A.] Argonne Natl Lab, Nucl Engn Div, Argonne, IL 60439 USA. RP Cammi, A (reprint author), Politecn Milan, Nucl Engn Div CeSNEF, Dept Energy, Via La Masa 34, I-20156 Milan, Italy. EM stefano.lorenzi@mail.polimi.it; antonio.cammi@polimi.it; sara.bortot@mail.polimi.it; roberto.ponciroli@mail.polimi.it; amoissey@anl.gov OI Cammi, Antonio/0000-0003-1508-5935 NR 19 TC 3 Z9 3 U1 0 U2 4 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0029-5493 J9 NUCL ENG DES JI Nucl. Eng. Des. PD JAN PY 2013 VL 254 BP 67 EP 88 DI 10.1016/j.nucengdes.2012.09.001 PG 22 WC Nuclear Science & Technology SC Nuclear Science & Technology GA 090TF UT WOS:000315002200008 ER PT J AU Ozaltun, H Shen, MHH Medvedev, P Miller, SJ AF Ozaltun, Hakan Shen, M. -H. Herman Medvedev, Pavel Miller, Samuel J. TI Computational evaluation for the mechanical behavior of U10Mo fuel mini plates subject to thermal cycling SO NUCLEAR ENGINEERING AND DESIGN LA English DT Article ID CREEP AB Mechanical behavior of the monolithic mini-plates during a post-fabrication furnace annealing was investigated. Monolithic fuel is a proposed fuel form to accomplish higher uranium densities in the reactor core and thermal cycling is a standard performance evaluation procedure for these fuel elements. To evaluate the mechanical performance of the plate under a thermal loading, a thermo-mechanical finite element simulation was performed. All three stages of the thermal cycling process were considered: (1) heating of a newly fabricated plate to 500 degrees C, (2) holding at a constant temperature of 500 degrees C for 60 min, and finally (3) cooling the plate to room temperature. Fabrication induced residual stress fields were implemented as the initial state for the thermal cycle model. It was shown that the fuel foil remains in the elastic regime during the entire process, while the cladding material exhibits additional plasticity. In particular, simulations have revealed the existence of a critical temperature at which the net stress fields on the fuel foils change directions. This stress reversal occurs between 400 and 450 degrees C which matches the experimental blister temperature of irradiated plates. It was shown that the fuel foil would be in fully tensile state above this transition temperature, facilitating the initiation of blisters. Long transverse edges and the regions around the corners of the fuel foil were identified as possible blister locations. The results have implied that a higher post-fabrication compressive stress field of the foil yields higher threshold temperatures; however, each thermal cycle would progressively relieve compressive stresses of the foil. Comparison with experiments has shown agreement, thus substantiated the capability of the model. (C) 2012 Elsevier B.V. All rights reserved. C1 [Ozaltun, Hakan; Shen, M. -H. Herman] Ohio State Univ, Dept Mech & Aerosp Engn, Scott Lab N350, Columbus, OH 43210 USA. [Ozaltun, Hakan; Medvedev, Pavel; Miller, Samuel J.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. RP Ozaltun, H (reprint author), Idaho Natl Lab, POB 1625, Idaho Falls, ID 83415 USA. EM Hakan.Ozaltun@inl.gov OI Ozaltun, Hakan/0000-0002-9975-2506 FU US Department of Energy [DE-AC07-05ID14517]; agency of the U.S. Government FX This manuscript has been authored under Contract No. DE-AC07-05ID14517 with the US Department of Energy. The US Government retains and the publisher, by accepting the article for publication, acknowledges that the US Government retains a nonexclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for US Government purposes.; This information was prepared as an account of work sponsored by an agency of the U.S. Government. Neither the U.S. Government nor any agency thereof, nor any of their employees, makes any warranty, express or implied, or assumes any legal liability or responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would not infringe privately owned rights. References herein to any specific commercial product, process, or service by trade name, trademark, manufacturer, or otherwise, does not necessarily constitute or imply its endorsement, recommendation, or favoring by the U.S. Government or any agency thereof. The views and opinions of authors expressed herein do not necessarily state or reflect those of the U.S. Government or any agency thereof. NR 22 TC 4 Z9 4 U1 1 U2 10 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0029-5493 EI 1872-759X J9 NUCL ENG DES JI Nucl. Eng. Des. PD JAN PY 2013 VL 254 BP 165 EP 178 DI 10.1016/j.nucengdes.2012.09.008 PG 14 WC Nuclear Science & Technology SC Nuclear Science & Technology GA 090TF UT WOS:000315002200017 ER PT J AU Sakamoto, Y Garnier, JC Rouault, J Grandy, C Fanning, T Hill, R Chikazawa, Y Kotake, S AF Sakamoto, Yoshihiko Garnier, Jean-Claude Rouault, Jacques Grandy, Christopher Fanning, Thomas Hill, Robert Chikazawa, Yoshitaka Kotake, Shoji TI Selection of sodium coolant for fast reactors in the US, France and Japan SO NUCLEAR ENGINEERING AND DESIGN LA English DT Article AB The joint paper presents a common view of fast reactor specific missions in the, development of nuclear energy and a cross-analysis of merits and demerits of several Fast Reactors concepts studied worldwide and especially in the Generation-IV International Forum (GIF) framework. The paper provides the context for fast reactors development in the United States, France and Japan and focuses on the comparison on Sodium-cooled Fast Reactor (SFR), Gas-cooled Fast Reactor (GFR), and Lead-cooled Fast Reactor (LFR), i.e. the three fast reactor concepts that have the potential to meet the nuclear fuel cycle sustainability goals. The information provided in the article permits the reader to understand each country's objectives to see that not only the objectives searched for but also the technical orientations are converging. The authors underline that SFR technology evaluation relies significantly on the substantial base technology development programs within each country which is without comparison for the other two fast reactor technologies, e.g.. SFR technology has already been developed to commercial or near commercial scale in each country whereas the performance of LFR and GFR technology is still uncertain. The main GFR merits are the potential for high temperatures and the easier possibilities for inspections and repairs. The main challenges are the fuel (fabrication, in-pile behavior), materials for high temperatures, and the implementation of mitigation means to manage severe core degradation. The main LFR merit is the lack of chemical reactivity of the lead coolant with air and water. The main challenges are the development of corrosion resistant structural and cladding materials, the implementation of mitigation means to manage severe core degradation, the density of the lead, and the comparably large core size. The selection of a reference fast reactor concept in view of possible industrialization is made on a national base, taking into account the each countries' strategic objectives, existing technology base, the proven or expected technical performance, the R&D challenges and technical means to conduct that R&D, the possibility to share development costs and risks, etc. It is important to note that in different contexts, the U.S., French, and Japanese organizations have selected the SFR as their reference fast reactor concept. (C) 2012 Elsevier BM. All rights reserved. C1 [Sakamoto, Yoshihiko; Chikazawa, Yoshitaka; Kotake, Shoji] Japan Atom Energy Agcy, Adv Nucl Syst Res & Dev Directorate, Oarai, Ibaraki 3111393, Japan. [Garnier, Jean-Claude; Rouault, Jacques] CEA, DEN, DER, Ctr Cadarache, F-13108 Saint Paul Lez Durance C, France. [Grandy, Christopher; Fanning, Thomas; Hill, Robert] Argonne Natl Lab, Nucl Engn Div, Argonne, IL 60439 USA. RP Sakamoto, Y (reprint author), Japan Atom Energy Agcy, Adv Nucl Syst Res & Dev Directorate, 4002 Narita Cho, Oarai, Ibaraki 3111393, Japan. EM sakamoto.yoshihiko@jaea.go.jp NR 43 TC 1 Z9 1 U1 1 U2 18 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0029-5493 J9 NUCL ENG DES JI Nucl. Eng. Des. PD JAN PY 2013 VL 254 BP 194 EP 217 DI 10.1016/j.nucengdes.2012.09.009 PG 24 WC Nuclear Science & Technology SC Nuclear Science & Technology GA 090TF UT WOS:000315002200020 ER PT J AU Yan, FY Lartey, M Damodaran, K Albenze, E Thompson, RL Kim, J Haranczyk, M Nulwala, HB Luebke, DR Smit, B AF Yan, Fangyong Lartey, Michael Damodaran, Krishnan Albenze, Erik Thompson, Robert L. Kim, Jihan Haranczyk, Maciej Nulwala, Hunaid B. Luebke, David R. Smit, Berend TI Understanding the effect of side groups in ionic liquids on carbon-capture properties: a combined experimental and theoretical effort SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID MOLECULAR-DYNAMICS METHOD; ATOM FORCE-FIELD; CO2 CAPTURE; DIFFUSION MEASUREMENTS; STIMULATED ECHO; GAS SOLUBILITY; NMR-DIFFUSION; SIMULATION; GRADIENT; DIOXIDE AB Ionic liquids are an emerging class of materials with applications in a variety of fields. Steady progress has been made in the creation of ionic liquids tailored to specific applications. However, the understanding of the underlying structure-property relationships has been slower to develop. As a step in the effort to alleviate this deficiency, the influence of side groups on ionic liquid properties has been studied through an integrated approach utilizing synthesis, experimental determination of properties, and simulation techniques. To achieve this goal, a classical force field in the framework of OPLS/Amber force fields has been developed to predict ionic liquid properties accurately. Cu(I)-catalyzed click chemistry was employed to synthesize triazolium-based ionic liquids with diverse side groups. Values of densities were predicted within 3% of experimental values, whereas self-diffusion coefficients were underestimated by about an order of magnitude though the trends were in excellent agreement, the activation energy calculated in simulation correlates well with experimental values. The predicted Henry coefficient for CO2 solubility reproduced the experimentally observed trends. This study highlights the importance of integrating experimental and computational approaches in property prediction and materials development, which is not only useful in the development of ionic liquids for CO2 capture but has application in many technological fields. C1 [Yan, Fangyong; Smit, Berend] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Yan, Fangyong; Kim, Jihan; Smit, Berend] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Lartey, Michael; Damodaran, Krishnan; Albenze, Erik; Thompson, Robert L.; Nulwala, Hunaid B.; Luebke, David R.] Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. [Damodaran, Krishnan] Univ Pittsburgh, Dept Chem, Pittsburgh, PA 15260 USA. [Albenze, Erik; Thompson, Robert L.] URS Corp, South Pk, PA 15219 USA. [Nulwala, Hunaid B.] Carnegie Mellon Univ, Dept Chem, Pittsburgh, PA 15213 USA. [Haranczyk, Maciej] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, Berkeley, CA 94720 USA. RP Nulwala, HB (reprint author), Natl Energy Technol Lab, POB 10940, Pittsburgh, PA 15236 USA. EM hnulwala@andrew.cmu.edu; david.luebke@netl.doe.gov; Berend-Smit@Berkeley.edu RI Smit, Berend/B-7580-2009; EFRC, CGS/I-6680-2012; Kim, Jihan/H-8002-2013; Haranczyk, Maciej/A-6380-2014; Nulwala, Hunaid/G-8126-2012; Stangl, Kristin/D-1502-2015 OI Smit, Berend/0000-0003-4653-8562; Haranczyk, Maciej/0000-0001-7146-9568; Nulwala, Hunaid/0000-0001-7481-3723; FU United States Department of Energy's Office of Fossil Energy under the National Energy Technology Laboratory [Car Cap_FY131415]; U.S. Department of Energy [DE-AC02-05CH11231]; Center for Gas Separations Relevant to Clean Energy Technologies, an Energy Frontier Research Center; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001015]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; Department of Energy, National Energy Technology Laboratory, an agency of the United States Government through URS Energy & Construction, Inc. FX ML, KD, EA, RLT, HBN, and DRL gratefully acknowledge the financial support by the United States Department of Energy's Office of Fossil Energy under the National Energy Technology Laboratory Field Work Proposal Car Cap_FY131415. FY and JK are supported by the Assistant Secretary for Fossil Energy of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. MH and B.S. were supported as part of the Center for Gas Separations Relevant to Clean Energy Technologies, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number DE-SC0001015. Berkeley Lab is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. We thank Li-Chiang Lin for helping to prepare the figures. This project was funded by the Department of Energy, National Energy Technology Laboratory, an agency of the United States Government, through a support contract with URS Energy & Construction, Inc. Neither the United States Government nor any agency thereof, nor any of their employees, nor URS Energy & Construction, Inc., nor any of their employees, makes any warranty, expressed or implied, or assumes any legal liability or responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would not infringe privately owned rights. Reference herein to any specific commercial product, process, or service by trade name, trademark, manufacturer, or otherwise, does not necessarily constitute or imply its endorsement, recommendation, or favoring by the United States Government or any agency thereof. The views and opinions of authors expressed herein do not necessarily state or reflect those of the United States Government or any agency thereof. NR 46 TC 16 Z9 16 U1 2 U2 90 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PY 2013 VL 15 IS 9 BP 3264 EP 3272 DI 10.1039/c3cp43923b PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 085ZD UT WOS:000314651900030 PM 23348234 ER PT J AU Pilli, SK Deutsch, TG Furtak, TE Brown, LD Turner, JA Herring, AM AF Pilli, Satyananda Kishore Deutsch, Todd G. Furtak, Thomas E. Brown, Logan D. Turner, John A. Herring, Andrew M. TI BiVO4/CuWO4 heterojunction photoanodes for efficient solar driven water oxidation SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID VISIBLE-LIGHT IRRADIATION; PHOTOELECTROCHEMICAL PROPERTIES; HYDROGEN-PRODUCTION; COPPER TUNGSTATE; SINGLE-CRYSTALS; THIN-FILMS; BIVO4; CATALYST; WO3; DECOMPOSITION AB BiVO4/CuWO4 heterojunction electrodes were prepared using spray deposition of a highly porous bismuth vanadate film onto the surface of an electrodeposited three dimensional network connected copper tungstate. Bilayer BiVO4/CuWO4/fluorine doped tin oxide glass (FTO) electrodes demonstrated higher photocurrent magnitudes than either with BiVO4/FTO or CuWO4/FTO electrodes in 1.0 M Na2SO4 electrolyte buffered at pH 7. The photocurrent is enhanced by the formation of the heterojunction that aids charge carrier collection brought about by the band edge offsets. When the pH 7 buffered electrolytes contained 1.0 M bicarbonate is employed instead of 1.0 M sulfate, the charge transfer resistance was decreased. This led to nearly 1.8 times the photocurrent density at 1.0 V vs. Ag/AgCl. The photocurrent was stable over 24 hours in bicarbonate electrolyte. C1 [Pilli, Satyananda Kishore; Brown, Logan D.; Herring, Andrew M.] Colorado Sch Mines, Dept Chem & Biol Engn, Golden, CO 80401 USA. [Deutsch, Todd G.; Turner, John A.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Furtak, Thomas E.] Colorado Sch Mines, Dept Phys, Golden, CO 80401 USA. RP Herring, AM (reprint author), Colorado Sch Mines, Dept Chem & Biol Engn, Golden, CO 80401 USA. EM spilli@mines.edu; aherring@mines.edu RI Brown, Logan/E-7699-2011; OI Deutsch, Todd/0000-0001-6577-1226; Herring, Andrew/0000-0001-7318-5999 FU Center for Revolutionary Solar Photoconversion FX We thank the Center for Revolutionary Solar Photoconversion for a seed grant. NR 39 TC 50 Z9 50 U1 12 U2 231 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PY 2013 VL 15 IS 9 BP 3273 EP 3278 DI 10.1039/c2cp44577h PG 6 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 085ZD UT WOS:000314651900031 PM 23348367 ER PT J AU Chang, C Tantawi, S Church, S Neilson, J Larkoski, PV AF Chang, Chao Tantawi, Sami Church, Sarah Neilson, Jeffery Larkoski, Patricia V. TI NOVEL COMPACT WAVEGUIDE DUAL CIRCULAR POLARIZER SO PROGRESS IN ELECTROMAGNETICS RESEARCH-PIER LA English DT Article ID ORTHOMODE TRANSDUCER; ANTENNA; DESIGN; SEPTUM AB A novel type of dual circular polarizer for simultaneously receiving and transmitting right-hand and left-hand circularly polarized waves is developed and tested. It consists of a H-plane T junction of rectangular waveguide, one circular waveguide as an E-plane arm located on top of the junction, and two metallic pins used for matching. The theoretical analysis and design of the three-physical-port and four-mode polarizer were researched by solving scattering-Matrix of the network and using a full-wave electromagnetic simulation tool. The optimized polarizer has the advantages of a very compact size with a volume smaller than 0.6 lambda(3), low complexity and manufacturing cost. A couple of the polarizer has been manufactured and tested, and the experimental results are basically consistent with the theories. C1 [Chang, Chao; Tantawi, Sami; Neilson, Jeffery] Stanford Univ, Stanford Linear Accelerator Ctr, Natl Accelerator Lab, Stanford, CA 94309 USA. [Chang, Chao; Church, Sarah; Larkoski, Patricia V.] Stanford Univ, Kavli Inst Particle Astrophys & Cosmol, Stanford, CA 94309 USA. [Church, Sarah; Larkoski, Patricia V.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Chang, Chao] Tsinghua Univ, Dept Engn Phys, Beijing 100084, Peoples R China. RP Chang, C (reprint author), Stanford Univ, Stanford Linear Accelerator Ctr, Natl Accelerator Lab, Stanford, CA 94309 USA. EM chang@slac.stanford.edu FU Department of Energy [DE-AC02-76SF00515] FX This work is supported by Department of Energy contract DE-AC02-76SF00515. NR 29 TC 8 Z9 8 U1 0 U2 9 PU E M W PUBLISHING PI CAMBRIDGE PA PO BOX 425517, KENDALL SQUARE, CAMBRIDGE, MA 02142 USA SN 1559-8985 J9 PROG ELECTROMAGN RES JI Prog. Electromagn. Res. PY 2013 VL 136 BP 1 EP 16 PG 16 WC Engineering, Electrical & Electronic; Physics, Applied; Telecommunications SC Engineering; Physics; Telecommunications GA 087FY UT WOS:000314747900001 ER PT J AU Wall, NA Karunathilake, N Dong, W AF Wall, N. A. Karunathilake, N. Dong, W. TI Interactions of Tc(IV) with citrate in NaCl media SO RADIOCHIMICA ACTA LA English DT Article DE Technetium; Citrate; Complexation; Solvent extraction; PHREEQC ID HIGH IONIC-STRENGTH; METAL-LIGAND INTERACTIONS; TECHNETIUM REDUCTION; STABILITY-CONSTANTS; OXALATE COMPLEXES; BEHAVIOR; DOUNREAY; ACETATE; FE(II); SYSTEM AB This paper presents the experimental determination of the stability constant for the citrate complexes with TcO(OH)(+) and TcO(OH)(2)(0) at different ionic strengths (NaCl), using a solvent extraction method. Data show that the stability constants for the formation of TcO(OH)Cit(2-) and TcO(OH)(2)Cit(3-) are 10(7.5+/-0.2) and 10(2.8+/-0.2) respectively, at zero ionic strength, with an average of 10(6.5+/-0.3) and 10(2.8+/-0.2) respectively, in the 1.0-3.0 M ionic strength range. PHREEQC calculations based on these stability constants show that the TcO(OH)Cit(2-) is the predominant species between pH 3 and 8 and that 50 mM citrate leads to a Tc(IV) solubility of 2x10(-5) M at pH 5. C1 [Wall, N. A.; Karunathilake, N.] Washington State Univ, Dept Chem, Pullman, WA 99164 USA. [Dong, W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Wall, NA (reprint author), Washington State Univ, Dept Chem, Pullman, WA 99164 USA. EM nawall@wsu.edu RI Dong, Wenming/G-3221-2015 OI Dong, Wenming/0000-0003-2074-8887 FU Office of the Biological and Environmental Research, Office of Science, U.S. Department of Energy (DOE) [DE-FG02-08ER64696]; Washington State University; U.S. Nuclear Regulatory Commission [3808953] FX This work was supported by the Office of the Biological and Environmental Research, Office of Science, U.S. Department of Energy (DOE) under the grant DE-FG02-08ER64696 with Washington State University and by the U.S. Nuclear Regulatory Commission under the grant 3808953. NR 34 TC 4 Z9 4 U1 2 U2 14 PU OLDENBOURG VERLAG PI MUNICH PA LEKTORAT MINT, POSTFACH 80 13 60, D-81613 MUNICH, GERMANY SN 0033-8230 J9 RADIOCHIM ACTA JI Radiochim. Acta PY 2013 VL 101 IS 2 BP 111 EP 116 DI 10.1524/ract.2013.2001 PG 6 WC Chemistry, Inorganic & Nuclear; Nuclear Science & Technology SC Chemistry; Nuclear Science & Technology GA 093GE UT WOS:000315178900006 ER PT J AU Carmichael, JR Diallo, SO AF Carmichael, J. R. Diallo, S. O. TI A cryogenic high pressure cell for inelastic neutron scattering measurements of quantum fluids and solids SO REVIEW OF SCIENTIFIC INSTRUMENTS LA English DT Article ID MOMENTUM DISTRIBUTION; HELIUM AB We present our new development of a high pressure cell for inelastic neutron scattering measurements of helium at ultra-low temperatures. The cell has a large sample volume of similar to 140 cm(3) and a working pressure of similar to 7MPa, with a relatively thin wall-thickness (1.1 mm)-thanks to the high yield strength aluminum used in the design. Two variants of this cell have been developed. The first cell is permanently joined components using electron-beam welding and explosion welding, methods that have little or no impact on the global heat treatment of the cell. The second cell discussed has modular and interchangeable components, which includes a capacitance pressure gauge, that can be sealed using the traditional indium wire technique. The performance of the cells have been tested in recent measurements on superfluid liquid helium near the solidification line. (C) 2013 American Institute of Physics. [http://dx.doi.org/10.1063/1.4772764] C1 [Carmichael, J. R.] Oak Ridge Natl Lab, Instrument & Source Design Div, Oak Ridge, TN 37831 USA. [Diallo, S. O.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. RP Carmichael, JR (reprint author), Oak Ridge Natl Lab, Instrument & Source Design Div, Oak Ridge, TN 37831 USA. EM carmichaeljr@ornl.gov; omardiallosl@ornl.gov RI Diallo, Souleymane/B-3111-2016; BL18, ARCS/A-3000-2012 OI Diallo, Souleymane/0000-0002-3369-8391; FU Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy (DOE) FX We thank the sample environment group at the Spallation Neutron Source (SNS) for their valuable technical support. We are grateful to Jacques Bossy of Insititut Neel (French National Center for Scientific Research (CNRS)) for his helpful advice regarding the design of the pressure transducer and Mark Rennich and Ken Herwig of the SNS for a critical reading of this article. This research at Oak Ridge National Laboratory's Spallation Neutron Source, was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy (DOE). NR 20 TC 0 Z9 0 U1 2 U2 17 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0034-6748 EI 1089-7623 J9 REV SCI INSTRUM JI Rev. Sci. Instrum. PD JAN PY 2013 VL 84 IS 1 AR 015101 DI 10.1063/1.4772764 PG 7 WC Instruments & Instrumentation; Physics, Applied SC Instruments & Instrumentation; Physics GA 086ZH UT WOS:000314729100060 PM 23387689 ER PT J AU Fredenburg, DA Koller, DD Rigg, PA Scharff, RJ AF Fredenburg, D. A. Koller, D. D. Rigg, P. A. Scharff, R. J. TI High-fidelity Hugoniot analysis of porous materials SO REVIEW OF SCIENTIFIC INSTRUMENTS LA English DT Article ID SHOCK COMPRESSION; HIGH-PRESSURE; DYNAMIC COMPACTION; POWDER COMPACTION; STATE; ALUMINUM; EQUATION; COPPER; IRON; WAVE AB An experimental technique and analysis methodology for obtaining high-fidelity Hugoniot measurements with defined uncertainty bounds on powder compacts using optical velocimetry is presented. Impedance matching is used to calculate the shocked state in the powder from the measured initial compact density, rho(00), impact velocity, V-Imp, and shock velocity, U-S. Detailed characterization of the powder thicknesses at precise locations results in improvements in characterization of the initial density state and accurate measurements of the powder thickness at locations corresponding to shock velocity measurements. These measurements result in high accuracies in the equilibrium Hugoniot state and reduced uncertainties in the measured and calculated Hugoniot parameters. Assumptions in this analysis include a constant and homogeneous initial porous density, and steady state wave propagation. The approach is applied to a system of CeO2 powder pressed to 4.0 g/cm(3) (55% theoretical maximum density), and results indicate a complex dynamic response. (C) 2013 American Institute of Physics. [http://dx.doi.org/10.1063/1.4774394] C1 [Fredenburg, D. A.; Koller, D. D.; Rigg, P. A.; Scharff, R. J.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Fredenburg, DA (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM dafreden@lanl.gov OI Scharff, Robert/0000-0002-1708-8964 FU National Nuclear Security Administration of the U.S. Department of Energy [DE-AC52-06NA25396] FX The authors would like to thank M. Byers, S. DiMarino, R. Manzanares, B. Bartram, A. Pacheco, and B. Nolen for target preparation, gas-gun operations, and materials characterization. This work was conducted at Los Alamos National Laboratory, an affirmative action/equal opportunity employer, which is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy under Contract No. DE-AC52-06NA25396. NR 41 TC 2 Z9 2 U1 3 U2 21 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0034-6748 J9 REV SCI INSTRUM JI Rev. Sci. Instrum. PD JAN PY 2013 VL 84 IS 1 AR 013903 DI 10.1063/1.4774394 PG 10 WC Instruments & Instrumentation; Physics, Applied SC Instruments & Instrumentation; Physics GA 086ZH UT WOS:000314729100035 PM 23387664 ER PT J AU Gaume, RM Lam, S Gascon, M Setyawan, W Curtarolo, S Feigelson, RS AF Gaume, R. M. Lam, S. Gascon, M. Setyawan, W. Curtarolo, S. Feigelson, R. S. TI An apparatus for studying scintillator properties at high isostatic pressures SO REVIEW OF SCIENTIFIC INSTRUMENTS LA English DT Article ID TRAPPED EXCITON LUMINESCENCE; ELECTRONIC BAND-STRUCTURES; HYDROSTATIC-PRESSURE; NON-PROPORTIONALITY; ENERGY RESOLUTION; UNIAXIAL-STRESS; TEMPERATURE; NONPROPORTIONALITY; NAI(TL); BGO AB We describe the design and operation of a unique hydraulic press for the study of scintillator materials under isostatic pressure. This press, capable of developing a pressure of a gigapascal, consists of a large sample chamber pressurized by a two-stage hydraulic amplifier. The optical detection of the scintillation light emitted by the sample is performed, through a large aperture optical port, by a photodetector located outside the pressure vessel. In addition to providing essential pressure-dependent studies on the emission characteristics of radioluminescent materials, this apparatus is being developed to elucidate the mechanisms behind the recently observed dependency of light-yield nonproportionality on electronic band structure. The variation of the light output of a Tl:CsI crystal under 511-keV gamma excitation and hydrostatic pressure is given as an example. (C) 2013 American Institute of Physics. [http://dx.doi.org/10.1063/1.4773563] C1 [Gaume, R. M.] Univ Cent Florida, Coll Opt & Photon CREOL, Orlando, FL 32816 USA. [Gaume, R. M.] Univ Cent Florida, NanoSci Technol Ctr, Orlando, FL 32816 USA. [Lam, S.; Gascon, M.; Feigelson, R. S.] Stanford Univ, Dept Mat Sci & Engn, Stanford, CA 94305 USA. [Setyawan, W.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Curtarolo, S.] Duke Univ, Dept Mech Engn & Mat Sci, Durham, NC 27708 USA. RP Gaume, RM (reprint author), Univ Cent Florida, Coll Opt & Photon CREOL, Orlando, FL 32816 USA. EM gaume@ucf.edu RI Gascon, Martin/C-9440-2011 OI Gascon, Martin/0000-0002-2065-009X FU Domestic Nuclear Defense Office (DNDO) [2008-DN-077-ARI005-02] FX The authors wish to thank W. Newhall of Harwood Engineering, Inc. and GTAT Crystal Systems, LLC for their helpful discussions. This work was supported by the Domestic Nuclear Defense Office (DNDO) under Grant No. 2008-DN-077-ARI005-02. NR 33 TC 0 Z9 0 U1 0 U2 11 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0034-6748 J9 REV SCI INSTRUM JI Rev. Sci. Instrum. PD JAN PY 2013 VL 84 IS 1 AR 015109 DI 10.1063/1.4773563 PG 6 WC Instruments & Instrumentation; Physics, Applied SC Instruments & Instrumentation; Physics GA 086ZH UT WOS:000314729100068 PM 23387697 ER PT J AU Jensen, BJ Owens, CT Ramos, KJ Yeager, JD Saavedra, RA Iverson, AJ Luo, SN Fezzaa, K Hooks, DE AF Jensen, B. J. Owens, C. T. Ramos, K. J. Yeager, J. D. Saavedra, R. A. Iverson, A. J. Luo, S. N. Fezzaa, K. Hooks, D. E. TI Impact system for ultrafast synchrotron experiments SO REVIEW OF SCIENTIFIC INSTRUMENTS LA English DT Article ID RAY-DIFFRACTION MEASUREMENTS; KCL AB The impact system for ultrafast synchrotron experiments, or IMPULSE, is a 12.6-mm bore light-gas gun (<1 km/s projectile velocity) designed specifically for performing dynamic compression experiments using the advanced imaging and X-ray diffraction methods available at synchrotron sources. The gun system, capable of reaching projectile velocities up to 1 km/s, was designed to be portable for quick insertion/removal in the experimental hutch at Sector 32 ID-B of the Advanced Photon Source (Argonne, IL) while allowing the target chamber to rotate for sample alignment with the beam. A key challenge in using the gun system to acquire dynamic data on the nanosecond time scale was synchronization (or bracketing) of the impact event with the incident X-ray pulses (80 ps width). A description of the basic gun system used in previous work is provided along with details of an improved launch initiation system designed to significantly reduce the total system time from launch initiation to impact. Experiments were performed to directly measure the gun system time and to determine the gun performance curve for projectile velocities ranging from 0.3 to 0.9 km/s. All results show an average system time of 21.6 +/- 4.5 ms, making it possible to better synchronize the gun system and detectors to the X-ray beam. (C) 2013 American Institute of Physics. [http://dx.doi.org/10.1063/1.4774389] C1 [Jensen, B. J.; Owens, C. T.; Ramos, K. J.; Yeager, J. D.; Saavedra, R. A.; Luo, S. N.; Hooks, D. E.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Iverson, A. J.] Natl Secur Technol, Los Alamos, NM 87544 USA. [Fezzaa, K.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Jensen, BJ (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM bjjensen@lanl.gov RI Luo, Sheng-Nian /D-2257-2010; OI Luo, Sheng-Nian /0000-0002-7538-0541; Yeager, John/0000-0002-3121-6053 FU LANL; National Security Technologies (NSTech) Shock Wave Physics Related Diagnostics (SWRD) program; Agnew National Security Fellowship; U.S. Department of Energy (DOE) [DE-AC52-06NA25396]; U.S. DOE [DE-AC02-06CH11357] FX This work was performed at Los Alamos National Laboratory and Argonne National Laboratory's Advanced Photon Source. Tim Pierce is gratefully acknowledged for his help in target and projectile fabrication, gun setup, and shot execution. A. Deriy (Argonne National Laboratory) is thanked for technical support at Sector 32 of the Advanced Photon Source and James Esparza is thanked for his technical support during the initial gun testing. C. Hall (Sandia National Laboratory) is thanked for providing the initial breech design for the launcher system. This work was supported by LANL's MaRIE and Science Campaign programs and National Security Technologies (NSTech) Shock Wave Physics Related Diagnostics (SWRD) program. J. D. Yeager was supported by the Agnew National Security Fellowship. LANL is operated by Los Alamos National Security, LLC for the U.S. Department of Energy (DOE) under Contract No. DE-AC52-06NA25396. Use of the Advanced Photon Source, an Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. NR 17 TC 10 Z9 10 U1 3 U2 39 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0034-6748 J9 REV SCI INSTRUM JI Rev. Sci. Instrum. PD JAN PY 2013 VL 84 IS 1 AR 013904 DI 10.1063/1.4774389 PG 5 WC Instruments & Instrumentation; Physics, Applied SC Instruments & Instrumentation; Physics GA 086ZH UT WOS:000314729100036 PM 23387665 ER PT J AU Moro, EA Briggs, ME AF Moro, Erik A. Briggs, Matthew E. TI Note: Simultaneous measurement of transverse speed and axial velocity from a single optical beam SO REVIEW OF SCIENTIFIC INSTRUMENTS LA English DT Article ID SPECKLE; VELOCIMETRY; DOPPLER AB A method is introduced for simultaneously measuring transverse speed and axial velocity using a single optical beam and a standard photon Doppler velocimetry (PDV) sensing architecture. This result is of particular interest given the recent, widespread use of PDV and the fact that optical velocimetry has thus far been limited to measuring motion in one dimension per probe. Further, this result demonstrates that both axial velocity data and transverse speed data (at least qualitative) may be obtained entirely through signal analysis; not requiring hardware modification. This result is immediately relevant to analyses of existing PDV data and to future efforts in high-speed optical velocimetry. (C) 2013 American Institute of Physics. [http://dx.doi.org/10.1063/1.4789764] C1 [Moro, Erik A.; Briggs, Matthew E.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Moro, EA (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. NR 9 TC 5 Z9 5 U1 1 U2 10 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0034-6748 J9 REV SCI INSTRUM JI Rev. Sci. Instrum. PD JAN PY 2013 VL 84 IS 1 AR 016110 DI 10.1063/1.4789764 PG 3 WC Instruments & Instrumentation; Physics, Applied SC Instruments & Instrumentation; Physics GA 086ZH UT WOS:000314729100087 PM 23387716 ER PT J AU Rodriguez, G Sandberg, RL McCulloch, Q Jackson, SI Vincent, SW Udd, E AF Rodriguez, G. Sandberg, R. L. McCulloch, Q. Jackson, S. I. Vincent, S. W. Udd, E. TI Chirped fiber Bragg grating detonation velocity sensing SO REVIEW OF SCIENTIFIC INSTRUMENTS LA English DT Article ID SHOCK DYNAMICS AB An all optical-fiber-based approach to measuring high explosive detonation front position and velocity is described. By measuring total light return using an incoherent light source reflected from a linearly chirped fiber Bragg grating sensor in contact with the explosive, dynamic mapping of the detonation front position and velocity versus time is obtained. We demonstrate two calibration procedures and provide several examples of detonation front measurements: PBX 9502 cylindrical rate stick, radial detonation front in PBX 9501, and PBX 9501 detonation along curved meridian line. In the cylindrical rate stick measurement, excellent agreement with complementary diagnostics (electrical pins and streak camera imaging) is achieved, demonstrating accuracy in the detonation front velocity to below the 0.3% level when compared to the results from the pin data. Finally, an estimate on the linear spatial and temporal resolution of the system shows that sub-mm and sub-mu s levels are attainable with proper consideration of the recording speed, detection sensitivity, spectrum, and chirp properties of the grating. (C) 2013 American Institute of Physics. [http://dx.doi.org/10.1063/1.4774112] C1 [Rodriguez, G.; Sandberg, R. L.; McCulloch, Q.] Los Alamos Natl Lab, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA. [Jackson, S. I.; Vincent, S. W.] Los Alamos Natl Lab, Weapons Expt Div, Los Alamos, NM 87545 USA. [Udd, E.] Columbia Gorge Res, Fairview, OR 97024 USA. RP Rodriguez, G (reprint author), Los Alamos Natl Lab, Mat Phys & Applicat Div, POB 1663, Los Alamos, NM 87545 USA. EM rodrigeo@lanl.gov RI Rodriguez, George/G-7571-2012; OI Rodriguez, George/0000-0002-6044-9462; Jackson, Scott/0000-0002-6814-3468; Sandberg, Richard/0000-0001-9719-8188 FU Gemini Project; Campaign 2 "High Explosive Science" Program at Los Alamos National Laboratory under Department of Energy [DE-AC52-06NA25396] FX Funding for this work was provided by the Gemini Project and the Campaign 2 "High Explosive Science" Program at Los Alamos National Laboratory under the auspices of the Department of Energy for Los Alamos National Security LLC under Contract No. DE-AC52-06NA25396. The authors also thank the Center for Integrated Nanotechnologies, Los Alamos National Laboratory for providing access to their ultrafast laser machining facility to cut and calibrate the fiber Bragg gratings used in this work. The authors also recognize M. Shinas of Los Alamos National Laboratory and V. Romero of National Security Technologies, Inc. for technical support on initial demonstration experiments. Also, M. Furlanetto of Los Alamos National Laboratory is acknowledged for program support under the Gemini Project at Los Alamos National Laboratory. NR 17 TC 11 Z9 12 U1 0 U2 30 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0034-6748 J9 REV SCI INSTRUM JI Rev. Sci. Instrum. PD JAN PY 2013 VL 84 IS 1 AR 015003 DI 10.1063/1.4774112 PG 10 WC Instruments & Instrumentation; Physics, Applied SC Instruments & Instrumentation; Physics GA 086ZH UT WOS:000314729100054 PM 23387683 ER PT J AU Saunders, A Makela, M Bagdasarova, Y Back, HO Boissevain, J Broussard, LJ Bowles, TJ Carr, R Currie, SA Filippone, B Garcia, A Geltenbort, P Hickerson, KP Hill, RE Hoagland, J Hoedl, S Holley, AT Hogan, G Ito, TM Lamoreaux, S Liu, CY Liu, J Mammei, RR Martin, J Melconian, D Mendenhall, MP Morris, CL Mortensen, RN Pattie, RW Pitt, M Plaster, B Ramsey, J Rios, R Sallaska, A Seestrom, SJ Sharapov, EI Sjue, S Sondheim, WE Teasdale, W Young, AR VornDick, B Vogelaar, RB Wang, Z Xu, YP AF Saunders, A. Makela, M. Bagdasarova, Y. Back, H. O. Boissevain, J. Broussard, L. J. Bowles, T. J. Carr, R. Currie, S. A. Filippone, B. Garcia, A. Geltenbort, P. Hickerson, K. P. Hill, R. E. Hoagland, J. Hoedl, S. Holley, A. T. Hogan, G. Ito, T. M. Lamoreaux, Steve Liu, Chen-Yu Liu, J. Mammei, R. R. Martin, J. Melconian, D. Mendenhall, M. P. Morris, C. L. Mortensen, R. N. Pattie, R. W., Jr. Pitt, M. Plaster, B. Ramsey, J. Rios, R. Sallaska, A. Seestrom, S. J. Sharapov, E. I. Sjue, S. Sondheim, W. E. Teasdale, W. Young, A. R. VornDick, B. Vogelaar, R. B. Wang, Z. Xu, Yanping TI Performance of the Los Alamos National Laboratory spallation-driven solid-deuterium ultra-cold neutron source SO REVIEW OF SCIENTIFIC INSTRUMENTS LA English DT Article ID LIFETIME MEASUREMENT; MAMBO II; REACTOR; STORAGE; RATES; UCN AB In this paper, we describe the performance of the Los Alamos spallation-driven solid-deuterium ultra-cold neutron (UCN) source. Measurements of the cold neutron flux, the very low energy neutron production rate, and the UCN rates and density at the exit from the biological shield are presented and compared to Monte Carlo predictions. The cold neutron rates compare well with predictions from the Monte Carlo code MCNPX and the UCN rates agree with our custom UCN Monte Carlo code. The source is shown to perform as modeled. The maximum delivered UCN density at the exit from the biological shield is 52(9) UCN/cc with a solid deuterium volume of similar to 1500 cm(3). (C) 2013 American Institute of Physics. [http://dx.doi.org/10.1063/1.4770063] C1 [Saunders, A.; Makela, M.; Bagdasarova, Y.; Boissevain, J.; Bowles, T. J.; Currie, S. A.; Hill, R. E.; Hogan, G.; Ito, T. M.; Lamoreaux, Steve; Morris, C. L.; Mortensen, R. N.; Ramsey, J.; Seestrom, S. J.; Sjue, S.; Sondheim, W. E.; Teasdale, W.; Wang, Z.] Los Alamos Natl Lab, Los Alamos, NM 87544 USA. [Back, H. O.; Broussard, L. J.; Hoagland, J.; Holley, A. T.; Pattie, R. W., Jr.; Young, A. R.; VornDick, B.; Xu, Yanping] N Carolina State Univ, Dept Phys, Raleigh, NC 27695 USA. [Carr, R.; Filippone, B.; Hickerson, K. P.; Ito, T. M.; Liu, J.; Martin, J.; Mendenhall, M. P.] CALTECH, Kellogg Radiat Lab, Pasadena, CA 91125 USA. [Garcia, A.; Hoedl, S.; Sallaska, A.; Sjue, S.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Geltenbort, P.] Inst Laue Langevin, F-38042 Grenoble 9, France. [Lamoreaux, Steve] Yale Univ, Dept Phys, New Haven, CT 06520 USA. [Liu, Chen-Yu] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Liu, J.] Shanghai Jiao Tong Univ, Dept Phys, Shanghai 200240, Peoples R China. [Mammei, R. R.; Pitt, M.; Vogelaar, R. B.] Virginia Tech, Dept Phys, Blacksburg, VA 24061 USA. [Martin, J.] Univ Winnipeg, Winnipeg, MB R3B 2E9, Canada. [Melconian, D.] Texas A&M Univ, Inst Cyclotron, College Stn, TX 77843 USA. [Plaster, B.] Univ Kentucky, Dept Phys & Astron, Lexington, KY 40506 USA. [Rios, R.] Idaho State Univ, Dept Phys, Pocatello, ID 83209 USA. [Sharapov, E. I.] Joint Inst Nucl Res, Dubna 141980, Russia. RP Saunders, A (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87544 USA. RI Melconian, Dan/A-1331-2011; Xu, Yanping /E-8437-2013; OI Melconian, Dan/0000-0002-0142-5428; Broussard, Leah/0000-0001-9182-2808; Makela, Mark/0000-0003-0592-3683; Currie, Scott/0000-0002-6164-7321; Morris, Christopher/0000-0003-2141-0255; Ito, Takeyasu/0000-0003-3494-6796; Garcia, Alejandro/0000-0001-6056-6645 NR 44 TC 26 Z9 26 U1 1 U2 29 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0034-6748 J9 REV SCI INSTRUM JI Rev. Sci. Instrum. PD JAN PY 2013 VL 84 IS 1 AR 013304 DI 10.1063/1.4770063 PG 10 WC Instruments & Instrumentation; Physics, Applied SC Instruments & Instrumentation; Physics GA 086ZH UT WOS:000314729100010 PM 23387639 ER PT J AU Taubman, MS AF Taubman, Matthew S. TI Note: Switch-mode hybrid current controllers for quantum cascade lasers SO REVIEW OF SCIENTIFIC INSTRUMENTS LA English DT Article AB Chemical sensing in the mid-infrared has been revolutionized by the advent of quantum cascade lasers. Their higher current and voltage demands compared to laser diodes however, negatively impact size, weight, and power footprint for fieldable systems, particularly in hot environments. This Note presents a switch-mode/linear hybrid controller, furnishing drive currents up to 2 A at compliance voltages up to 15 V, with output noise near levels determined by shot and Johnson contributions from within the linear regulator, from frequencies below 100 Hz to the switching frequency. Current modulation from near 0 to 1.8 A is also demonstrated at frequencies up to a kilohertz. (C) 2013 American Institute of Physics. [http://dx.doi.org/10.1063/1.4774046] C1 Pacific NW Natl Lab, Richland, WA 99352 USA. RP Taubman, MS (reprint author), Pacific NW Natl Lab, POB 999, Richland, WA 99352 USA. EM Matthew.Taubman@pnnl.gov FU Battelle Memorial Institute [DE-AC06-76RLO 1830]; (U.S.) Department of Energy (DOE) office of Nonproliferation and Verification Research and Development [NA-22] FX The author wishes to thank Bret Cannon for useful discussions, and Rob Stahl for board layout and prototype construction. The Pacific Northwest National Laboratory (PNNL) is operated for the U.S. Department of Energy by the Battelle Memorial Institute under Contract No. DE-AC06-76RLO 1830. The work at PNNL was supported in part by the (U.S.) Department of Energy (DOE) office of Nonproliferation and Verification Research and Development, NA-22. NR 4 TC 2 Z9 2 U1 1 U2 12 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0034-6748 J9 REV SCI INSTRUM JI Rev. Sci. Instrum. PD JAN PY 2013 VL 84 IS 1 AR 016103 DI 10.1063/1.4774046 PG 3 WC Instruments & Instrumentation; Physics, Applied SC Instruments & Instrumentation; Physics GA 086ZH UT WOS:000314729100080 PM 23387709 ER PT J AU Wang, CL Clonts, LG Diawara, Y Hannan, BW Hodges, JP AF Wang, C. L. Clonts, L. G. Diawara, Y. Hannan, B. W. Hodges, J. P. TI Elimination of ghosting artifacts from wavelength-shifting fiber neutron detectors SO REVIEW OF SCIENTIFIC INSTRUMENTS LA English DT Article AB Misassignment of neutron position (ghosting) produces artifacts which have been observed in wavelength-shifting (WLS) fiber detectors developed for time-of-flight (TOF) neutron powder diffraction. In position-sensitive detectors (PSDs) with WLS fiber encoding, thermal and cold neutrons interact with a monolithic (LiF)-Li-6/ZnS:Ag scintillator screen, and scintillation photons are generated and transported through the crossed fibers to photomultipliers (PMTs). The neutron position is determined by photon counts in the PMTs within a preset time window. Ghosting occurs when neutrons hit the group boundaries of two neighboring PMTs for x-position multiplexing, which is modeled as resulting from a long travel length (about 3-5 mm) of a small number of scintillation photons. This model is supported by the change observed in aperture images when the threshold number for photon-pulses was adjusted for neutron event determination. When the threshold number of photon-pulses was set above 10 for each PMT, the ghost peaks in the aperture images and TOF spectra of powder diffraction were strongly suppressed or completely eliminated, and the intrinsic background levels of the WLS detectors were significantly reduced. Our result indicates that WLS fiber detector is a promising alternative for He-3 PSDs for neutron scattering. (C) 2013 American Institute of Physics. [http://dx.doi.org/10.1063/1.4789497] C1 [Wang, C. L.; Diawara, Y.; Hannan, B. W.; Hodges, J. P.] Oak Ridge Natl Lab, Instrument & Source Design Div, Neutron Sci Directorate, Oak Ridge, TN 37831 USA. [Clonts, L. G.] Oak Ridge Natl Lab, Res Accelerator Div, Neutron Sci Directorate, Oak Ridge, TN 37831 USA. RP Wang, CL (reprint author), Oak Ridge Natl Lab, Instrument & Source Design Div, Neutron Sci Directorate, Oak Ridge, TN 37831 USA. EM wangc@ornl.gov RI Hodges, Jason/K-1421-2013; OI Wang, Cai-Lin/0000-0001-9745-2334 FU UT-Batelle, LLC [DE-AC05-00OR22725]; U.S. Department of Energy FX We acknowledge much help and discussion with R. Cooper, L. Crow, A. Ke, R. Riedel, L. Robertson, and H. D. Skorpenske, and comments on the manuscript made by K. W. Herwig (ORNL). We would like to thank C. Kline and H. E. Workman (PartTec Ltd., Bloomington, IN) for their dedication in detector fabrication. This work was supported by UT-Batelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. NR 13 TC 2 Z9 2 U1 0 U2 17 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0034-6748 EI 1089-7623 J9 REV SCI INSTRUM JI Rev. Sci. Instrum. PD JAN PY 2013 VL 84 IS 1 AR 013308 DI 10.1063/1.4789497 PG 6 WC Instruments & Instrumentation; Physics, Applied SC Instruments & Instrumentation; Physics GA 086ZH UT WOS:000314729100014 PM 23387643 ER PT J AU Wen, H Wolfe, DE Gomella, AA Miao, HX Xiao, XH Liu, CA Lynch, SK Morgan, N AF Wen, Han Wolfe, Douglas E. Gomella, Andrew A. Miao, Houxun Xiao, Xianghui Liu, Chian Lynch, Susanna K. Morgan, Nicole TI Interferometric hard x-ray phase contrast imaging at 204 nm grating period SO REVIEW OF SCIENTIFIC INSTRUMENTS LA English DT Article ID FABRICATION AB We report on hard x-ray phase contrast imaging experiments using a grating interferometer of approximately 1/10th the grating period achieved in previous studies. We designed the gratings as a staircase array of multilayer stacks which are fabricated in a single thin film deposition process. We performed the experiments at 19 keV x-ray energy and 0.8 mu m pixel resolution. The small grating period resulted in clear separation of different diffraction orders and multiple images on the detector. A slitted beam was used to remove overlap of the images from the different diffraction orders. The phase contrast images showed detailed features as small as 10 mu m, and demonstrated the feasibility of high resolution x-ray phase contrast imaging with nanometer scale gratings. (C) 2013 American Institute of Physics. [http://dx.doi.org/10.1063/1.4788910] C1 [Wen, Han; Gomella, Andrew A.; Miao, Houxun; Lynch, Susanna K.] NHLBI, Imaging Phys Lab, Biophys & Biochem Ctr, NIH, Bethesda, MD 20892 USA. [Wolfe, Douglas E.] Penn State Univ, Appl Res Lab, State Coll, PA 16804 USA. [Xiao, Xianghui; Liu, Chian] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. [Morgan, Nicole] Natl Inst Biomed Imaging & Bioengn, NIH, Bethesda, MD 20892 USA. RP Wen, H (reprint author), NHLBI, Imaging Phys Lab, Biophys & Biochem Ctr, NIH, Bldg 10, Bethesda, MD 20892 USA. EM wenh@nhlbi.nih.gov RI Miao, Houxun/N-8233-2013; Wen, Han/G-3081-2010 OI Wen, Han/0000-0001-6844-2997 FU Division of Intramural Research, National Heart, Lung and Blood Institute, National Institutes of Health [HL006143-01]; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX We thank Eric Bennett and Dr. Dumitru Mazilu of the National Institutes of Health (NIH) for their assistance with grating fabrication and imager assembly. We thank Cliff Sonnenbrot and Dr. Alan Michelson of NIH for assistance with fruit flies. The grating substrates were made at the Nanofab Facility of the National Institute of Standards and Technology. The work was funded by the Division of Intramural Research, National Heart, Lung and Blood Institute, National Institutes of Health, under Project No. HL006143-01. Use of the Advanced Photon Source at Argonne National Laboratory was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 22 TC 5 Z9 5 U1 0 U2 19 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0034-6748 J9 REV SCI INSTRUM JI Rev. Sci. Instrum. PD JAN PY 2013 VL 84 IS 1 AR 013706 DI 10.1063/1.4788910 PG 5 WC Instruments & Instrumentation; Physics, Applied SC Instruments & Instrumentation; Physics GA 086ZH UT WOS:000314729100029 PM 23387658 ER PT J AU Zheng, XY Deotte, J Alonso, MP Farquar, GR Weisgraber, TH Gemberling, S Lee, H Fang, N Spadaccini, CM AF Zheng, Xiaoyu Deotte, Joshua Alonso, Matthew P. Farquar, George R. Weisgraber, Todd H. Gemberling, Steven Lee, Howon Fang, Nicholas Spadaccini, Christopher M. TI Design and optimization of a light-emitting diode projection micro-stereolithography three-dimensional manufacturing system (vol 83, 125001, 2012) SO REVIEW OF SCIENTIFIC INSTRUMENTS LA English DT Correction C1 [Zheng, Xiaoyu; Deotte, Joshua; Alonso, Matthew P.; Farquar, George R.; Weisgraber, Todd H.; Gemberling, Steven; Spadaccini, Christopher M.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Alonso, Matthew P.] Univ Illinois, Dept Mech Sci & Engn, Urbana, IL 61801 USA. [Lee, Howon; Fang, Nicholas] MIT, Dept Mech Engn, Cambridge, MA 02139 USA. RP Zheng, XY (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RI Fang, Nicholas/A-5856-2008; OI Fang, Nicholas/0000-0001-5713-629X; Zheng, Xiaoyu/0000-0001-8685-5728 NR 1 TC 0 Z9 0 U1 5 U2 28 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0034-6748 J9 REV SCI INSTRUM JI Rev. Sci. Instrum. PD JAN PY 2013 VL 84 IS 1 AR 019902 DI 10.1063/1.4773408 PG 1 WC Instruments & Instrumentation; Physics, Applied SC Instruments & Instrumentation; Physics GA 086ZH UT WOS:000314729100089 ER PT J AU Pandey, A Prasad, A Moscatello, JP Engelhard, M Wang, CM Yap, YK AF Pandey, Archana Prasad, Abhishek Moscatello, Jason P. Engelhard, Mark Wang, Chongmin Yap, Yoke Khin TI Very Stable Electron Field Emission from Strontium Titanate Coated Carbon Nanotube Matrices with Low Emission Thresholds SO ACS NANO LA English DT Article DE carbon nanotubes; strontium titanate; poly(methyl methacrylate); field emission ID ARRAYS; SRTIO3; FILMS AB Novel PMMA-STO-CNT matrices were created by I opened-tip vertically aligned multiwalled carbon nanotubes (VA-MWCNTs) with conformal coatings of strontium titanate (STO) and poly(methyl methacrylate) (PMMA). Emission threshold of 0.8 V/mu m was demonstrated, about 5-fold lower than that of the as-grown VA-MWCNTs. This was obtained after considering the related band structures under the perspective of work functions and tunneling width as a function of the STO thickness. We showed that there is an optimum thickness of STO coatings to effectively reduce the work function of CNTs and yet minimize the tunneling width for electron emissions. Furthermore, simulation and modeling suggest that PMMA-STO-CNT matrices have suppressed screening effects and Coulombs' repulsion forces between electrons in adjacent CNTs, leading to low emission threshold, high emission density, and prolonged emission stability. These findings are important for practical application of VA-MWCNTs In field emission devices, X-ray generation, and wave amplification. C1 [Pandey, Archana; Prasad, Abhishek; Moscatello, Jason P.; Yap, Yoke Khin] Michigan Technol Univ, Dept Phys, Houghton, MI 49931 USA. [Engelhard, Mark; Wang, Chongmin] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. RP Yap, YK (reprint author), Michigan Technol Univ, Dept Phys, 118 Fisher Hall,1400 Townsend Dr, Houghton, MI 49931 USA. EM ykyap@mtu.edu OI Moscatello, Jason/0000-0003-0043-4709; Yap, Yoke Khin/0000-0002-1224-4120; Engelhard, Mark/0000-0002-5543-0812 FU Defense Advanced Research Projects Agency [DAAD17-03-C-0115]; U.S. Department of Army [W911NF-04-1-0029]; Department of Energy's Office of Biological and Environmental Research located at Pacific Northwest National Laboratory FX This work was supported by the Defense Advanced Research Projects Agency (Contract No. DAAD17-03-C-0115 through the U.S. Army Research Laboratory), and the U.S. Department of Army (Grant No. W911NF-04-1-0029 through the City College of New York). Part of the sample characterization was performed at the Environmental Molecular Sciences Laboratory, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research located at Pacific Northwest National Laboratory. NR 28 TC 22 Z9 22 U1 1 U2 68 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 J9 ACS NANO JI ACS Nano PD JAN PY 2013 VL 7 IS 1 BP 117 EP 125 DI 10.1021/nn303351g PG 9 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 078FB UT WOS:000314082800016 PM 23199078 ER PT J AU Zhang, XW Yazyev, OV Feng, JJ Xie, LM Tao, CG Chen, YC Jiao, LY Pedramrazi, Z Zettl, A Louie, SG Dai, HJ Crommie, MF AF Zhang, Xiaowei Yazyev, Oleg V. Feng, Juanjuan Xie, Liming Tao, Chenggang Chen, Yen-Chia Jiao, Liying Pedramrazi, Zahra Zettl, Alex Louie, Steven G. Dai, Hongjie Crommie, Michael F. TI Experimentally Engineering the Edge Termination of Graphene Nanoribbons SO ACS NANO LA English DT Article DE graphene nanoribbon; synthesis; scanning tunneling microscopy; first-principles calculations ID STATES; PSEUDOPOTENTIALS; GRAPHITE AB The edges of graphene nanoribbons (GNRs) have attracted much interest due to their potentially strong influence on GNR electronic and magnetic properties. Here we report the ability to engineer the microscopic edge termination of high-quality GNRs via hydrogen plasma etching. Using a combination of high-resolution scanning tunneling microscopy and first-principles calculations, we have determined the exact atomic structure of plasma-etched GNR edges and established the chemical nature of terminating functional groups for zigzag, armchair, and chiral edge orientations. We find that the edges of hydrogen-plasma-etched GNRs are generally flat, free of structural reconstructions, and terminated by hydrogen atoms with no rehybridlzation of the outermost carbon edge atoms. Both zigzag and chiral edges show the presence of edge states. C1 [Zhang, Xiaowei; Yazyev, Oleg V.; Feng, Juanjuan; Tao, Chenggang; Chen, Yen-Chia; Pedramrazi, Zahra; Zettl, Alex; Louie, Steven G.; Crommie, Michael F.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Zhang, Xiaowei; Yazyev, Oleg V.; Tao, Chenggang; Chen, Yen-Chia; Zettl, Alex; Louie, Steven G.; Crommie, Michael F.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Yazyev, Oleg V.] Ecole Polytech Fed Lausanne EPFL, Inst Theoret Phys, CH-1015 Lausanne, Switzerland. [Feng, Juanjuan] Lanzhou Univ, Sch Phys Sci & Technol, Lanzhou 730000, Gansu, Peoples R China. [Xie, Liming; Jiao, Liying; Dai, Hongjie] Stanford Univ, Dept Chem, Stanford, CA 94305 USA. [Xie, Liming; Jiao, Liying; Dai, Hongjie] Stanford Univ, Adv Mat Lab, Stanford, CA 94305 USA. RP Crommie, MF (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM crommie@berkeley.edu RI Yazyev, Oleg/A-4073-2008; Xie, Liming/C-4639-2011; Jiao, Liying/C-6307-2011; Zettl, Alex/O-4925-2016 OI Yazyev, Oleg/0000-0001-7281-3199; Zettl, Alex/0000-0001-6330-136X FU Office of Naval Research Multidisciplinary University Research Initiative (MURI) [N00014-09-1-1066]; Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231]; National Science Foundation [DMR10-1006184]; Swiss National Science Foundation [PP00P2_133552]; Samsung; MARCO MSD FX Research supported by the Office of Naval Research Multidisciplinary University Research Initiative (MURI) Award No. N00014-09-1-1066 (GNR sample preparation and characterization, thermodynamic stability calculation), by the Director, Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231 (STM instrumentation development and development of numerical simulation tools), and by National Science Foundation Award No. DMR10-1006184 (calculation of theoretical LDOS). O.V.Y. acknowledges support from the Swiss National Science Foundation Grant No. PP00P2_133552 (development of new techniques for edge simulation). L.X., L.J., and H.D. acknowledge support from Samsung and MARCO MSD (development of nanoribbons synthesis and plasma etching). NR 28 TC 79 Z9 80 U1 10 U2 276 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 J9 ACS NANO JI ACS Nano PD JAN PY 2013 VL 7 IS 1 BP 198 EP 202 DI 10.1021/nn303730v PG 5 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 078FB UT WOS:000314082800024 PM 23194280 ER PT J AU Kamcev, J Germack, DS Nykypanchuk, D Grubbs, RB Nam, CY Black, CT AF Kamcev, Jovan Germack, David S. Nykypanchuk, Dmytro Grubbs, Robert B. Nam, Chang-Yong Black, Charles T. TI Chemically Enhancing Block Copolymers for Block-Selective Synthesis of Self-Assembled Metal Oxide Nanostructures SO ACS NANO LA English DT Article DE block copolymers; infiltration synthesis; atomic layer deposition; metal oxides; photo-oxidation ID ATOMIC LAYER DEPOSITION; SEQUENTIAL INFILTRATION SYNTHESIS; SEPARATED DIBLOCK COPOLYMER; OPTICAL LITHOGRAPHY; HYBRID MATERIALS; THIN-FILMS; X-RAY; POLYSTYRENE; CHEMISTRY; ULTRAVIOLET AB We report chemical modification of self-assembled block copolymer thin films by ultraviolet light that enhances the block-selective affinity of organometallic precursors otherwise lacking preference for either copolymer block. Sequential precursor loading and reaction facilitate formation of zinc oxide, titanium dioxide, and aluminum oxide nanostructures within the polystyrene domains of both lamellar- and cylindrical-phase modified polystyrene-block-poly(methyl methacrylate) thin film templates. Near-edge X-ray absorption fine structure measurements and Fourier transform infrared spectroscopy show that photo-oxidation by ultraviolet light creates Lewis basic groups within polystyrene, resulting in an increased Lewis base acid interaction with the organometallic precursors. The approach provides a method for generating both aluminum oxide patterns and their corresponding inverses using the same block copolymer template. C1 [Kamcev, Jovan; Nykypanchuk, Dmytro; Grubbs, Robert B.; Nam, Chang-Yong; Black, Charles T.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Germack, David S.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RP Nam, CY (reprint author), Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. EM cynam@bnl.gov; ctblack@bnl.gov RI Paquette, Joseph/O-4271-2015; Nam, Chang-Yong/D-4193-2009; OI Paquette, Joseph/0000-0001-6023-5125; Nam, Chang-Yong/0000-0002-9093-4063; Kamcev, Jovan/0000-0003-0379-5171 FU U.S. Department of Energy, Basic Energy Sciences, at the Center for Functional Nanomaterials; Materials Sciences and Engineering Division [DE AC02 98CH10886]; Energy Laboratory Research and Development Initiative at Brookhaven National Laboratory FX This research is supported by the U.S. Department of Energy, Basic Energy Sciences, at the Center for Functional Nanomaterials (J.K., D.N., R.B.G., C.-Y.N., and C.T.B.) and the Materials Sciences and Engineering Division (D.S.G.) (Contract No. DE AC02 98CH10886). This work was partially supported by the Energy Laboratory Research and Development Initiative at Brookhaven National Laboratory. The authors thank Dr. Mingzhao Liu for helpful discussion. NR 46 TC 21 Z9 21 U1 4 U2 86 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 J9 ACS NANO JI ACS Nano PD JAN PY 2013 VL 7 IS 1 BP 339 EP 346 DI 10.1021/nn304122b PG 8 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 078FB UT WOS:000314082800038 PM 23252934 ER PT J AU Robinson, JT Schmucker, SW Diaconescu, CB Long, JP Culbertson, JC Ohta, T Friedman, AL Beechem, TE AF Robinson, Jeremy T. Schmucker, Scott W. Diaconescu, C. Bogdan Long, James P. Culbertson, James C. Ohta, Taisuke Friedman, Adam L. Beechem, Thomas E. TI Electronic Hybridization of Large-Area Stacked Graphene Films SO ACS NANO LA English DT Article DE twisted bilayer graphene; interlayer coupling; absorption; functionalization ID CHEMICAL-VAPOR-DEPOSITION; BILAYER GRAPHENE; LAYERS; HETEROSTRUCTURES; GROWTH; CARBON AB Direct, tunable coupling between individually assembled graphene layers is a next step toward designer two-dimensional (2D) crystal systems, with relevance for fundamental studies and technological applications. Here we describe the fabrication and characterization of large-area (>cm(2)), coupled bilayer graphene on SiO2/Si substrates. Stacking two graphene films leads to direct electronic interactions between layers, where the resulting film properties are determined by the local twist angle. Polycrystalline bilayer films have a "stained-glass window" appearance explained by the emergence of a narrow absorption band in the visible spectrum that depends on twist angle. Direct measurement of layer orientation via electron diffraction, together with Raman and optical spectroscopy, confirms the persistence of clean interfaces over large areas. Finally, we demonstrate that interlayer coupling can be reversibly turned off through chemical modification, enabling optical-based chemical detection schemes. Together, these results suggest that 2D crystals can be individually assembled to form electronically coupled systems suitable for large-scale applications. C1 [Robinson, Jeremy T.; Schmucker, Scott W.; Long, James P.; Culbertson, James C.; Friedman, Adam L.] USN, Res Lab, Washington, DC 20007 USA. [Diaconescu, C. Bogdan; Ohta, Taisuke; Beechem, Thomas E.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Robinson, JT (reprint author), USN, Res Lab, Washington, DC 20007 USA. EM jeremy.robinson@nrl.navy.mil RI Friedman, Adam/D-9610-2011; Robinson, Jeremy/F-2748-2010; Schmucker, Scott/D-8312-2012 OI Friedman, Adam/0000-0003-0597-5432; Schmucker, Scott/0000-0003-2908-5282 FU Office of Naval Research; NRL's Nanoscience Institute; National Research Council; U.S. DOE Office of Basic Energy Sciences (BES), Division of Materials Science and Engineering; Sandia LDRD; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The work at the Naval Research Laboratory was supported by the Office of Naval Research and NRL's Nanoscience Institute. J.T.R. is grateful for continued technical support from D. Zapotok and D. St Amand and C.D. Cress for assistance with Graphic Design. This research was performed while S.W.S held a National Research Council Research Associateship Award at the Naval Research Laboratory. The work at Sandia National Laboratories was supported by the U.S. DOE Office of Basic Energy Sciences (BES), Division of Materials Science and Engineering and by Sandia LDRD. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL85000. NR 51 TC 34 Z9 34 U1 6 U2 80 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 EI 1936-086X J9 ACS NANO JI ACS Nano PD JAN PY 2013 VL 7 IS 1 BP 637 EP 644 DI 10.1021/nn304834p PG 8 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 078FB UT WOS:000314082800067 PM 23240977 ER PT J AU Kang, YJ Pyo, JB Ye, XC Diaz, RE Gordon, TR Stach, EA Murray, CB AF Kang, Yijin Pyo, Jun Beom Ye, Xingchen Diaz, Rosa E. Gordon, Thomas R. Stach, Eric A. Murray, Christopher B. TI Shape-Controlled Synthesis of Pt Nanocrystals: The Role of Metal Carbonyls SO ACS NANO LA English DT Article DE platinum; nanocrystal; shape control; morphology; catalysis; electrocatalysis; CO oxidation ID PLATINUM SINGLE-CRYSTALS; CUBIC FE NANOPARTICLES; HIGH-INDEX FACETS; STRUCTURE SENSITIVITY; SUPERLATTICE MEMBRANES; PALLADIUM ICOSAHEDRA; ATMOSPHERIC-PRESSURE; CHEMICAL-SYNTHESIS; TWINNED STRUCTURE; OXYGEN REDUCTION AB Well-controlled synthesis of nanocrystals is necessary to unambiguously correlate the structural properties of nanocrystals with the catalytic properties. The most common low-index surfaces are (111) and (100). Therefore, model materials with {111} and {100} facets are highly desirable, in order to understand the catalytic properties of (111) and (100) surfaces for various structure-sensitive reactions. We report a solution-phase synthesis using metal carbonyls as additives. This synthetic method produces highly monodisperse Pt octahedra and icosahedra as the model of Pt{111}, Pt cubes as the model of Pt{100}, respectively. Several other morphologies, such as truncated cubes, cuboctahedra, spheres, tetrapods, star-shaped octapods, multipods, and hyper-branched structure, are produced, as well. A bifunctional role of metal carbonyl in the synthesis is identified: zerovalent transition metal decomposed from metal carbonyl acts as a shape-directing agent, while CO provides the reducing power. These high-quality shape-controlled Pt nanocrystals are suitable for model catalyst studies. C1 [Kang, Yijin; Ye, Xingchen; Gordon, Thomas R.; Murray, Christopher B.] Univ Penn, Dept Chem, Philadelphia, PA 19104 USA. [Pyo, Jun Beom; Murray, Christopher B.] Univ Penn, Dept Mat Sci & Engn, Philadelphia, PA 19104 USA. [Diaz, Rosa E.; Stach, Eric A.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Murray, CB (reprint author), Univ Penn, Dept Chem, Philadelphia, PA 19104 USA. EM cbmurray@sas.upenn.edu RI Stach, Eric/D-8545-2011; Gordon, Thomas/H-2924-2012; Kang, Yijin/E-7767-2012; Ye, Xingchen/D-3202-2017 OI Stach, Eric/0000-0002-3366-2153; Ye, Xingchen/0000-0001-6851-2721 FU National Science Foundation MRSEC [DMR11-20901]; Rachleff Scholars Program; Office of Naval Research (ONR) Multidisciplinary University Research Initiative (MURI) on Optical Metamaterials [N00014-10-1-0942]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX C.B.M. and Y.J.K. acknowledge the partial support from the National Science Foundation MRSEC DMR11-20901. J.P. acknowledges the support by the Rachleff Scholars Program. X.Y. acknowledges the support from the Office of Naval Research (ONR) Multidisciplinary University Research Initiative (MURI) on Optical Metamaterials through award N00014-10-1-0942. C.B.M. thanks the Richard Perry University Professorship for the support of his supervisor role. Research carried out in part at the Center for Functional Nanomaterials (CFN), Brookhaven National Laboratory (BNL), which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. We thank Charles Black (CFN, BNL) for the support at CFN, Douglas Yates at the Penn Regional Nanotechnology Facility for support in electron microscopy, and David Vann at Department of Earth and Environmental Science (University of Pennsylvania) for assistance in ICP-OES. NR 66 TC 57 Z9 57 U1 18 U2 290 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 J9 ACS NANO JI ACS Nano PD JAN PY 2013 VL 7 IS 1 BP 645 EP 653 DI 10.1021/nn3048439 PG 9 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 078FB UT WOS:000314082800068 PM 23211025 ER PT J AU Gu, M Belharouak, I Zheng, JM Wu, HM Xiao, J Genc, A Amine, K Thevuthasan, S Baer, DR Zhang, JG Browning, ND Liu, J Wang, CM AF Gu, Meng Belharouak, Ilias Zheng, Jianming Wu, Huiming Xiao, Jie Genc, Arda Amine, Khalil Thevuthasan, Suntharampillai Baer, Donald R. Zhang, Ji-Guang Browning, Nigel D. Liu, Jun Wang, Chongmin TI Formation of the Spinel Phase in the Layered Composite Cathode Used in Li-Ion Batteries SO ACS NANO LA English DT Article DE lithium ion battery; layered structure; spinel formation; phase transformation ID ELECTROCHEMICAL PERFORMANCE; LITHIUM BATTERIES; ELECTRON-MICROSCOPY; ANOMALOUS CAPACITY; OXIDE CATHODES; OXYGEN LOSS; STABILITY AB Pristine Li-rich layered cathodes, such as Li1.2Ni0.2Mn0.6O2 and Li1.2Ni0.1Mn0.525- Co0.175O2, were identified to exist in two different structures: LiMO2 R (3) over barm and LI2MO3 C2/m phases. Upon 300 cycles of charge/discharge, both phases gradually transform to the spinel structure. The transition from LiMO2 R (3) over barm to spinel is accomplished through the migration of transition metal ions to the Li site without breaking down the lattice, leading to the formation of mosaic structured spinel grains within the parent particle. In contrast, transition from Li2MO3 C2/m to spinel involves removal of Li+ and O2-, which produces large lattice strain and leads to the breakdown of the parent lattice. The newly formed spinel grains show random orientation within the same particle. Cracks and pores were also noticed within some layered nanoparticles after cycling, which is believed to be the consequence of the lattice breakdown and vacancy condensation upon removal of lithium ions. The AlF3-coating can partially relieve the spinel formation In the layered structure during cycling, resulting in a slower capacity decay. However, the AlF3-coating on the layered structure cannot ultimately stop the spinel formation. The observation of structure transition characteristics discussed in this paper provides direct explanation for the observed gradual capacity loss and poor rate performance of the layered composite. It also provides clues about how to improve the materials structure in order to Improve electrochemical performance. C1 [Gu, Meng; Thevuthasan, Suntharampillai; Baer, Donald R.; Wang, Chongmin] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Browning, Nigel D.; Liu, Jun] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. [Zheng, Jianming; Xiao, Jie; Zhang, Ji-Guang] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. [Belharouak, Ilias; Wu, Huiming; Amine, Khalil] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Genc, Arda] FEI Co, Hillsboro, OR 97124 USA. RP Wang, CM (reprint author), Pacific NW Natl Lab, Environm Mol Sci Lab, 902 Battelle Blvd, Richland, WA 99352 USA. EM Chongmin.Wang@pnnl.gov RI Baer, Donald/J-6191-2013; Amine, Khalil/K-9344-2013; Gu, Meng/B-8258-2013; Zheng, Jianming/F-2517-2014; OI Baer, Donald/0000-0003-0875-5961; Zheng, Jianming/0000-0002-4928-8194; Browning, Nigel/0000-0003-0491-251X; Belharouak, Ilias/0000-0002-3985-0278 FU U.S. Department of Energy (DOE) [DE-AC05-76RLO1830]; DOE's Office of Biological and Environmental Research; Office of Vehicle Technologies of DOE [AC02-05CH11231]; Office of Vehicle Technologies of DOE under Batteries for Advanced Transportation Technologies (BATT) program [18769]; DOE Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [KC020105-FWP12152]; DOE's Freedom CAR and Vehicle Technologies Office FX The research described in this paper is part of the Chemical Imaging Initiative at Pacific Northwest National Laboratory (PNNL). It was conducted under the Laboratory Directed Research and Development Program at PNNL, a multiprogram national laboratory operated by Battelle under Contract DE-AC05-76RLO1830 for the U.S. Department of Energy (DOE). The work was conducted in the William R. Wiley Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by DOE's Office of Biological and Environmental Research and located at PNNL. J. Zhang and J. Xiao would like to acknowledge the support of the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of DOE under Contract No. DE-AC02-05CH11231, Subcontract No. 18769 under the Batteries for Advanced Transportation Technologies (BATT) program. J. Liu would like to acknowledge the support of the DOE Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, under Award KC020105-FWP12152. I. Belharouak and K. Amine would like to acknowledge the support from DOE's Freedom CAR and Vehicle Technologies Office. NR 29 TC 243 Z9 248 U1 43 U2 562 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 J9 ACS NANO JI ACS Nano PD JAN PY 2013 VL 7 IS 1 BP 760 EP 767 DI 10.1021/nn305065u PG 8 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 078FB UT WOS:000314082800081 PM 23237664 ER PT J AU Choi, SJ Bennett, P Takei, K Wang, C Lo, CC Javey, A Bokor, J AF Choi, Sung-Jin Bennett, Patrick Takei, Kuniharu Wang, Chuan Lo, Cheuk Chi Javey, Ali Bokor, Jeffrey TI Short-Channel Transistors Constructed with Solution-Processed Carbon Nanotubes SO ACS NANO LA English DT Article DE carbon nanotubes; short channel; transistor; ballistic; solution-processed carbon nanotubes; contact resistance; quantum limit ID FIELD-EFFECT TRANSISTORS; OHMIC CONTACTS; ALIGNED ARRAYS; SEPARATION; ELECTRONICS; DIELECTRICS; CIRCUITS; MOBILITY AB We develop short-channel transistors using solution-processed single-walled carbon nanotubes (SWNTs) to evaluate the feasibility of those SWNTs for high-performance applications. Our results show that even though the intrinsic field-effect mobility is lower than the mobility of CVD nanotubes, the electrical contact between the nanotube and metal electrodes is not significantly affected. It is this contact resistance which often limits the performance of ultrascaled transistors. Moreover, we found that the contact resistance is lowered by the introduction of oxygen treatment. Therefore, high-performance solution-processed nanotube transistors with a 15 nm channel length were obtained by combining a top-gate structure and gate insulators made of a high-dielectric-constant ZrO2 film. The combination of these elements yields a performance comparable to that obtained with CVD nanotube transistors, which Indicates the potential for using solution-processed SWNTs for future aggressively scaled transistor technology. C1 [Bokor, Jeffrey] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. RP Bokor, J (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. EM jbokor@eecs.berkeley.edu RI Wang, Chuan/B-3649-2011; Javey, Ali/B-4818-2013; Foundry, Molecular/G-9968-2014; Bokor, Jeffrey/A-2683-2011 FU MSD Focus Center; Focus Center Research Program (FCRP); Semiconductor Research Corporation; DARPA/DSO Maximum Mobility and Manipulation FX This work was supported by the MSD Focus Center, one of six research centers funded under the Focus Center Research Program (FCRP), a Semiconductor Research Corporation entity and DARPA/DSO Maximum Mobility and Manipulation. NR 33 TC 35 Z9 35 U1 1 U2 81 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 J9 ACS NANO JI ACS Nano PD JAN PY 2013 VL 7 IS 1 BP 798 EP 803 DI 10.1021/nn305277d PG 6 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 078FB UT WOS:000314082800086 PM 23259742 ER PT J AU Zubelewicz, A Thompson, DG Ostoja-Starzewski, M Ionita, A Shunk, D Lewis, MW Lawson, JC Kale, S Koric, S AF Zubelewicz, Aleksander Thompson, Darla G. Ostoja-Starzewski, Martin Ionita, Axinte Shunk, Devin Lewis, Matthew W. Lawson, Joe C. Kale, Sohan Koric, Seid TI Fracture model for cemented aggregates SO AIP ADVANCES LA English DT Article ID CONSTITUTIVE MODEL; BRITTLE MATERIALS; UNIAXIAL TENSION; BEHAVIOR; STRESS; DAMAGE AB A mechanisms-based fracture model applicable to a broad class of cemented aggregates and, among them, plastic-bonded explosive (PBX) composites, is presented. The model is calibrated for PBX 9502 using the available experimental data under uniaxial compression and tension gathered at various strain rates and temperatures. We show that the model correctly captures inelastic stress-strain responses prior to the load peak and it predicts the post-critical macro-fracture processes, which result from the growth and coalescence of micro-cracks. In our approach, the fracture zone is embedded into elastic matrix and effectively weakens the material's strength along the plane of the dominant fracture. Copyright 2013 Author(s). This article is distributed under a Creative Commons Attribution 3.0 Unported License. [http://dx.doi.org/10.1063/1.4789791] C1 [Zubelewicz, Aleksander; Thompson, Darla G.; Ionita, Axinte; Shunk, Devin; Lewis, Matthew W.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Ostoja-Starzewski, Martin; Lawson, Joe C.; Kale, Sohan; Koric, Seid] Univ Illinois, Champaign, IL 61820 USA. RP Zubelewicz, A (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. OI Ostoja-Starzewski, Martin/0000-0002-3493-363X FU US Department of Energy; Enhanced Surveillance Program; Weapon Engineering Division, B61 Systems Program; NNSA of the U.S. DOE [DE-AC52-06NA25396] FX The authors wish to thank Racci DeLuca, WX-7, LANL, for her work on the HE mechanical testing. This project has been performed under the auspices of the US Department of Energy and was supported by the Enhanced Surveillance Program and the Weapon Engineering Division, B61 Systems Program. The Los Alamos National Laboratory is operated by Los Alamos National Security, LLC for the NNSA of the U.S. DOE under Contract No. DE-AC52-06NA25396. NR 16 TC 1 Z9 1 U1 2 U2 11 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 2158-3226 J9 AIP ADV JI AIP Adv. PD JAN PY 2013 VL 3 IS 1 AR 012119 DI 10.1063/1.4789791 PG 10 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA 086XH UT WOS:000314722300019 ER PT J AU Anderson, MD Heideman, CL Lin, QY Smeller, M Kokenyesi, R Herzing, AA Anderson, IM Keszler, DA Zschack, P Johnson, DC AF Anderson, Michael D. Heideman, Colby L. Lin, Qiyin Smeller, Mary Kokenyesi, Robert Herzing, Andrew A. Anderson, Ian M. Keszler, Douglas A. Zschack, Paul Johnson, David C. TI Size-Dependent Structural Distortions in One-Dimensional Nanostructures SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE chalcogenides; composites; hybrid materials; inorganic synthesis; nanomaterials ID BINARY NANOPARTICLE SUPERLATTICES; MISFIT LAYER COMPOUNDS; NANOCRYSTAL SUPERLATTICES; MONODISPERSE NANOCRYSTALS; SHAPE; ORGANIZATION; STABILITY; GOLD C1 [Anderson, Michael D.; Smeller, Mary; Johnson, David C.] Univ Oregon, Dept Chem, Eugene, OR 97403 USA. [Heideman, Colby L.] Eastern Oregon Univ, Dept Chem, La Grande, OR USA. [Lin, Qiyin] Univ Calif Irvine, Inst Telecommun & Informat Technol, Irvine, CA USA. [Kokenyesi, Robert; Keszler, Douglas A.] Oregon State Univ, Dept Chem, Corvallis, OR 97331 USA. [Herzing, Andrew A.; Anderson, Ian M.] NIST, Surface & Microanal Sci Div, Gaithersburg, MD 20899 USA. [Zschack, Paul] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Johnson, DC (reprint author), Univ Oregon, Dept Chem, Eugene, OR 97403 USA. EM davej@uoregon.edu OI Keszler, Douglas/0000-0002-7112-1171 FU National Science Foundation [DMR 0907049]; ONR [N00014-07-1-0358]; DGE [0549503]; National Science Foundation through CCI [CHE-1102637]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX The authors acknowledge support from the National Science Foundation through grant number DMR 0907049 and by ONR through grant number N00014-07-1-0358. Coauthors M. D. A. and C. L. H. acknowledge support from DGE (grant number 0549503). Coauthors R. K., D. A. K., and D.C.J. acknowledge support from the National Science Foundation through CCI grant number CHE-1102637. Use of the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under contract number DE-AC02-06CH11357. NR 21 TC 10 Z9 10 U1 2 U2 49 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1433-7851 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PY 2013 VL 52 IS 7 BP 1982 EP 1985 DI 10.1002/anie.201207825 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA 085ZY UT WOS:000314654000016 PM 23296571 ER PT J AU Oh, SJ Chun, W Riffat, SB Il Jeon, Y Dutton, S Han, HJ AF Oh, Seung Jin Chun, Wongee Riffat, Saffa B. Il Jeon, Young Dutton, Spencer Han, Hyun Joo TI Computational analysis on the enhancement of daylight penetration into dimly lit spaces: Light tube vs. fiber optic dish concentrator SO BUILDING AND ENVIRONMENT LA English DT Article DE Daylighting; Photometric analysis; Photopia; Radiance ID PERFORMANCE; BUILDINGS; ENERGY AB Capturing daylight into an unevenly lit lecture room with north-facing windows has been analyzed with the help of Photopia and Radiance. Two different daylighting systems, a light tube and a fiber-optic solar dish concentrator, are considered as means to lead light rays into an interior space with insufficient illumination from daylight. Photopia is used to photometrically model the daylighting systems as light travels through highly reflective light guiding elements of these systems. The candela power distribution curves (CDCs) generated by Photopia are imported by Radiance to produce photometric data and images of different locations in the lecture room. These results clearly reveal the functional benefits of each system when harvesting daylight for indoor illumination. For solar altitudes of less than 50 degrees, more daylight can be harvested by the solar tracking dish concentrator system. Also, its minimum-to-average (illuminance) uniformity ratio on the work plane remains between 0.55 and 0.72, varying quite less than that of the light tube, ranging from 0.46 to 0.88. (C) 2012 Published by Elsevier Ltd. C1 [Oh, Seung Jin; Chun, Wongee] Jeju Natl Univ, Dept Nucl & Energy Engn, Cheju 690756, South Korea. [Riffat, Saffa B.] Univ Nottingham, Dept Architecture & Built Environm, Nottingham NG7 2RD, England. [Il Jeon, Young] Dongguk Univ, Div Architectural Engn, Seoul 100715, South Korea. [Dutton, Spencer] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Han, Hyun Joo] Univ Nevada, Energy Res Ctr, Las Vegas, NV 89154 USA. RP Han, HJ (reprint author), Univ Nevada, Energy Res Ctr, Las Vegas, NV 89154 USA. EM HyunJoo.Han@unlv.edu FU National Research Foundation of Korea [2011-0029820] FX This work was partially sponsored by the National Research Foundation of Korea under Grant Number 2011-0029820. NR 19 TC 6 Z9 6 U1 0 U2 23 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-1323 J9 BUILD ENVIRON JI Build. Environ. PD JAN PY 2013 VL 59 BP 261 EP 274 DI 10.1016/j.buildenv.2012.08.025 PG 14 WC Construction & Building Technology; Engineering, Environmental; Engineering, Civil SC Construction & Building Technology; Engineering GA 082DG UT WOS:000314371900025 ER PT J AU Rees, SJ Haves, P AF Rees, Simon J. Haves, Philip TI An experimental study of air flow and temperature distribution in a room with displacement ventilation and a chilled ceiling SO BUILDING AND ENVIRONMENT LA English DT Article DE Displacement ventilation; Chilled ceiling; Convection; Room heat transfer; Air distribution ID NATURAL VENTILATION; THERMAL COMFORT; SYSTEMS; ENVIRONMENTS; CONVECTION; DESIGN; SPACES; PLUME; MODEL AB Displacement ventilation and chilled ceiling panel systems are potentially more energy efficient than conventional air conditioning systems and are characterized by the presence of vertical temperature gradients and significant radiant asymmetry. The characteristics of this type of system have been studied by making temperature and air flow measurements in a test chamber over a range of operating parameters typical of office applications. Results from the displacement ventilation study are consistent with other studies and show that normalized temperature profiles are independent of internal heat gain. Linear temperature gradients in the lower part of the room were found, in all cases, to be driven by convection from the adjacent walls. Significant mixing, indicated by reduced temperature gradients, was evident in the upper part of the room in the chilled ceiling results at higher levels of heat gain. Visualization experiments, velocity measurements and related numerical studies indicated that with greater heat gains the plumes have sufficient momentum to drive flow across the ceiling surface and down the walls. The significance of forced, as opposed to natural convection, is also suggested by relatively low Richardson Number (Ri) values found near the ceiling. Furthermore, in cases with moderately high internal gains, comparison of the temperature gradients indicated that the effect of ceiling surface temperature on the degree of mixing and the magnitude of the temperature gradient were of secondary importance. These findings are in contrast to the view that it is natural convection at the ceiling that causes enhanced mixing. (c) 2012 Elsevier Ltd. All rights reserved. C1 [Rees, Simon J.] De Montfort Univ, Inst Energy & Sustainable Dev, Leicester LE1 9BH, Leics, England. [Haves, Philip] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Rees, SJ (reprint author), De Montfort Univ, Inst Energy & Sustainable Dev, Leicester LE1 9BH, Leics, England. EM sjrees@dmu.ac.uk RI Rees, Simon/H-5517-2012; OI Rees, Simon/0000-0003-4869-1632 NR 47 TC 26 Z9 28 U1 1 U2 37 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-1323 J9 BUILD ENVIRON JI Build. Environ. PD JAN PY 2013 VL 59 BP 358 EP 368 DI 10.1016/j.buildenv.2012.09.001 PG 11 WC Construction & Building Technology; Engineering, Environmental; Engineering, Civil SC Construction & Building Technology; Engineering GA 082DG UT WOS:000314371900033 ER PT J AU Walker, IS Sherman, MH AF Walker, Iain S. Sherman, Max H. TI Effect of ventilation strategies on residential ozone levels SO BUILDING AND ENVIRONMENT LA English DT Article DE Ozone; Mechanical ventilation; Filtration; ASHRAE Standard 62.2; Infiltration; Simulation ID BUILDING-MATERIALS; DEPOSITION VELOCITIES; DECAY-RATES; INDOOR AIR; REMOVAL; PENETRATION; EXPOSURES AB Elevated outdoor ozone levels are associated with adverse health effects. Because people spend the vast majority of their time indoors, reduction in indoor levels of ozone of outdoor origin would lower population exposures and might also lead to a reduction in ozone-associated adverse health effects. In most buildings, indoor ozone levels are diminished with respect to outdoor levels to an extent that depends on surface reactions and on the degree to which ozone penetrates the building envelope. Ozone enters buildings from outdoors together with the airflows that are driven by natural and mechanical means, including deliberate ventilation used to reduce concentrations of indoor-generated pollutants. When assessing the effect of deliberate ventilation on occupant health one should consider not only the positive effects on removing pollutants of indoor origin but also the possibility that enhanced ventilation might increase indoor levels of pollutants originating outdoors. This study considers how changes in residential ventilation that are designed to comply with ASHRAE Standard 62.2 might influence indoor levels of ozone. Simulation results show that the building envelope can contribute significantly to filtration of ozone. Consequently, the use of exhaust ventilation systems is predicted to produce lower indoor ozone concentrations than would occur with balanced ventilation systems operating at the same air-exchange rate. We also investigated a strategy for reducing exposure to ozone that would deliberately reduce ventilation rates during times of high outdoor ozone concentration while still meeting daily average ventilation requirements. Published by Elsevier Ltd. C1 [Walker, Iain S.; Sherman, Max H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, EETD, Berkeley, CA 94720 USA. RP Walker, IS (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, EETD, MS 90R-3083,1 Cyclotron Rd, Berkeley, CA 94720 USA. EM ISWalker@lbl.gov FU California Energy Commission Public Interest Energy Research Program [CEC-500-02-004]; Energy Efficiency and Renewable Energy, Building Technologies Program, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the California Energy Commission Public Interest Energy Research Program award number CEC-500-02-004 and the Assistant Secretary for Energy Efficiency and Renewable Energy, Building Technologies Program, of the U.S. Department of Energy under contract No. DE-AC02-05CH11231. NR 33 TC 7 Z9 7 U1 6 U2 56 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-1323 EI 1873-684X J9 BUILD ENVIRON JI Build. Environ. PD JAN PY 2013 VL 59 BP 456 EP 465 DI 10.1016/j.buildenv.2012.09.013 PG 10 WC Construction & Building Technology; Engineering, Environmental; Engineering, Civil SC Construction & Building Technology; Engineering GA 082DG UT WOS:000314371900042 ER PT J AU Chen, XY Goff, GS Quiroz-Guzman, M Fagnant, DP Brennecke, JF Scott, BL Runde, W AF Chen, Xiao-Yan Goff, George S. Quiroz-Guzman, Mauricio Fagnant, Daniel P., Jr. Brennecke, Joan F. Scott, Brian L. Runde, Wolfgang TI Directed nucleation of monomeric and dimeric uranium(VI) complexes with a room temperature carboxyl-functionalized phosphonium ionic liquid SO CHEMICAL COMMUNICATIONS LA English DT Article ID METAL-COMPLEXES; OXIDES; U(VI); SALTS AB The carboxyl-functionalized phosphonium ionic liquid (IL), [HCTMP]-[Tf2N], enabled the directed nucleation of monomeric or dimeric uranyl(VI) compounds. This new IL is the first carboxyl-functionalized IL which is liquid at room temperature and exhibits a wider electro-chemical window and lower melting point than its ammonium analogue. C1 [Chen, Xiao-Yan; Goff, George S.] Los Alamos Natl Lab, Div Chem, Los Alamos, NM 87545 USA. [Quiroz-Guzman, Mauricio; Fagnant, Daniel P., Jr.; Brennecke, Joan F.] Univ Notre Dame, Dept Chem & Biomol Engn, Notre Dame, IN 46556 USA. [Scott, Brian L.] Los Alamos Natl Lab, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA. [Runde, Wolfgang] Los Alamos Natl Lab, Sci Program Off, Los Alamos, NM 87545 USA. RP Goff, GS (reprint author), Los Alamos Natl Lab, Div Chem, POB 1663, Los Alamos, NM 87545 USA. EM georgeg@lanl.gov; runde@lanl.gov RI Scott, Brian/D-8995-2017 OI Scott, Brian/0000-0003-0468-5396 FU Los Alamos Laboratory; G.T. Seaborg Institute for Transactinium Science at Los Alamos National Laboratory FX The authors gratefully acknowledge the Los Alamos Laboratory Directed Research and Development Program and the G.T. Seaborg Institute for Transactinium Science at Los Alamos National Laboratory for financial support. NR 21 TC 14 Z9 14 U1 0 U2 53 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1359-7345 J9 CHEM COMMUN JI Chem. Commun. PY 2013 VL 49 IS 19 BP 1903 EP 1905 DI 10.1039/c2cc38255e PG 3 WC Chemistry, Multidisciplinary SC Chemistry GA 086AM UT WOS:000314655400004 PM 23296265 ER PT J AU Ren, WS Lukens, WW Zi, GF Maron, L Walter, MD AF Ren, Wenshan Lukens, Wayne W. Zi, Guofu Maron, Laurent Walter, Marc D. TI Is the bipyridyl thorium metallocene a low-valent thorium complex? A combined experimental and computational study SO CHEMICAL SCIENCE LA English DT Article ID DECAMETHYLYTTERBOCENE COMPLEXES; TRIVALENT THORIUM; REACTIVITY; LANTHANIDE; LIGAND; BOND; TRIS(CYCLOPENTADIENYL)THORIUM(III); 2,2'-BIPYRIDYL; REDUCTION; CLEAVAGE AB Bipyridyl thorium metallocenes [eta(5)-1,2,4-(Me3C)(3)C5H2](2)Th(bipy) (1) and [eta(5)-1,3-(Me3C)(2)C5H3](2)Th(bipy) (2) have been investigated by magnetic susceptibility and computational studies. The magnetic susceptibility data reveal that 1 and 2 are not diamagnetic, but they behave as temperature independent paramagnets (TIPs). To rationalize this observation, density functional theory (DFT) and complete active space selfconsistent field (CASSCF) calculations have been undertaken, which indicated that Cp02Th(bipy) has indeed a Th(IV)(bipy(2-)) ground state (f(0)d(0)pi*(2), S = 0), but the open-shell singlet (f(0)d(1)pi*(1), S = 0) (almost degenerate with its triplet congener) is only 9.2 kcal mol(-1) higher in energy. Complexes 1 and 2 react cleanly with Ph2CS to give [eta(5)-1,2,4-(Me3C)(3)C5H2](2)Th[(bipy)(SCPh2)] (3) and [eta(5)-1,3-(Me3C)(2)C5H3](2)Th [(bipy)(SCPh2)] (4), respectively, in quantitative conversions. Since no intermediates were observed experimentally, this reaction was also studied computationally. Whereas coordination of Ph2CS to 2 in its S = 0 ground state is not possible, Ph2CS can coordinate to 2 in its triplet state (S = 1) upon which a single electron transfer (SET) from the (bipy(2-)) fragment to Ph2CS followed by C-C coupling takes place. C1 [Ren, Wenshan; Zi, Guofu] Beijing Normal Univ, Dept Chem, Beijing 100875, Peoples R China. [Ren, Wenshan] Southwest Univ, Coll Chem & Chem Engn, Chongqing 400715, Peoples R China. [Lukens, Wayne W.] Lawrence Berkeley Natl Lab, Actinide Chem Grp, Div Chem Sci, Berkeley, CA 94720 USA. [Maron, Laurent] Univ Toulouse, INSA, UPS, F-31077 Toulouse, France. [Maron, Laurent] LPCNO, CNRS, F-31077 Toulouse, France. [Walter, Marc D.] Tech Univ Carolo Wilhelmina Braunschweig, Inst Anorgan & Analyt Chem, D-38106 Braunschweig, Germany. RP Zi, GF (reprint author), Beijing Normal Univ, Dept Chem, Beijing 100875, Peoples R China. EM gzi@bnu.edu.cn; laurent.maron@irsamc.ups-tlse.fr; mwalter@tu-bs.de RI Walter, Marc/E-4479-2012 FU National Natural Science Foundation of China [20972018, 21074013, 21172022]; Program for New Century Excellent Talents in University [NCET-10-0253]; Fundamental Research Funds for the Central Universities (China); Deutsche Forschungsgemeinscha. (DFG) through the Emmy-Noether program [WA 2513/2-1]; Humboldt Foundation; U.S. Department of Energy, Basic Energy Sciences, Chemical Sciences, Biosciences, and Geosciences Division, Heavy Element Chemistry and were performed at Lawrence Berkeley National Laboratory [DE AC02 05CH11231] FX This work was supported by the National Natural Science Foundation of China (Grant no. 20972018, 21074013, 21172022), the Program for New Century Excellent Talents in University (NCET-10-0253), the Fundamental Research Funds for the Central Universities (China), and the Deutsche Forschungsgemeinscha. (DFG) through the Emmy-Noether program (WA 2513/2-1). LM thanks CINES and CalMip for the generous grant of computing time. LM is a member of the Institut Universitaire de France. The Humboldt Foundation is also acknowledged for an experienced researcher grant (LM). Portions of this work (WL) were supported by the U.S. Department of Energy, Basic Energy Sciences, Chemical Sciences, Biosciences, and Geosciences Division, Heavy Element Chemistry and were performed at Lawrence Berkeley National Laboratory under Contract no. DE AC02 05CH11231. We thank Professor Richard A. Andersen for helpful discussions. NR 34 TC 23 Z9 23 U1 6 U2 41 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2041-6520 J9 CHEM SCI JI Chem. Sci. PY 2013 VL 4 IS 3 BP 1168 EP 1174 DI 10.1039/c2sc22013j PG 7 WC Chemistry, Multidisciplinary SC Chemistry GA 083OR UT WOS:000314474900038 ER PT J AU Jones, MB Gaunt, AJ Gordon, JC Kaltsoyannis, N Neu, MP Scott, BL AF Jones, Matthew B. Gaunt, Andrew J. Gordon, John C. Kaltsoyannis, Nikolas Neu, Mary P. Scott, Brian L. TI Uncovering f-element bonding differences and electronic structure in a series of 1:3 and 1:4 complexes with a diselenophosphinate ligand SO CHEMICAL SCIENCE LA English DT Article ID SEGMENTED CONTRACTION SCHEME; PSEUDOPOTENTIAL BASIS-SETS; N-DONOR LIGAND; COORDINATION CHEMISTRY; TRIVALENT ACTINIDE; CRYSTAL-STRUCTURE; LANTHANIDE(III)/ACTINIDE(III) DIFFERENTIATION; DITHIOPHOSPHINIC ACIDS; LANTHANIDE CATIONS; CHALCOGEN BOND AB Understanding the bonding trends within, and the differences between, the 4f and 5f element series with soft donor atom ligands will aid elucidation of the fundamental origins of actinide (An) versus lanthanide (Ln) selectivity that is integral to many advanced nuclear fuel cycle separation concepts. One of the principal obstacles to acquiring such knowledge is the dearth of well characterized transuranic molecules that prevents the necessary comparison of 4f versus 5f coordination chemistry, electronic structure, and bonding. Reported herein is new chemistry of selenium analogues of dithiophosphinate actinide extractants. Ln(III) and An(III/IV) complexes with the diselenophosphinate [Se2PPh2](-) anion have been synthesized, structurally and spectroscopically characterized, and quantum chemical calculations performed on model compounds in which the phenyl rings have been replaced by methyl groups. The complexes [Ln(III)(Se2PPh2)(3)(THF)(2)] (Ln = La (1), Ce (2), Nd (3)), [La-III(Se2PPh2)(3)(MeCN)(2)] (4), [Pu-III(Se2PPh2)(3)(THF)(2)] (5), [Et4N][M-III(Se2PPh2)(4)] (M = Ce (6), Pu (7)), and [An(IV)(Se2PPh2)(4)] (An = U (8), Np (9)), represent the first f-element diselenophosphinates. In conjunction with the calculated models, complexes 1-9 were utilized to examine two important factors: firstly, bonding trends/differences between trivalent 4f and 5f cations of near identical ionic radii; secondly, bonding trend differences across the 5f series within the An(IV) oxidation state. Analysis of both experimental and computational data supports the conclusion of enhanced covalent bonding contributions in Pu-III-Se versus Ce-III-Se bonding, while differences between U-IV-Se and Np-IV-Se bonding is satisfactorily accounted for by changes in the strength of ionic interactions as a result of the increased positive charge density on Np-IV compared to U-IV ions. These findings improve understanding of soft donor ligand binding to the f-elements, and are of relevance to the design and manipulation of f-element extraction processes. C1 [Jones, Matthew B.; Gaunt, Andrew J.; Gordon, John C.] Los Alamos Natl Lab, Div Chem, Los Alamos, NM 87545 USA. [Kaltsoyannis, Nikolas] UCL, Dept Chem, London WC1H 0AJ, England. [Neu, Mary P.] Los Alamos Natl Lab, Weapons Program, Los Alamos, NM 87545 USA. [Scott, Brian L.] Los Alamos Natl Lab, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA. RP Gaunt, AJ (reprint author), Los Alamos Natl Lab, Div Chem, POB 1663, Los Alamos, NM 87545 USA. EM gaunt@lanl.gov; n.kaltsoyannis@ucl.ac.uk RI Scott, Brian/D-8995-2017; OI Scott, Brian/0000-0003-0468-5396; Kaltsoyannis, Nikolas/0000-0003-0293-5742; Gaunt, Andrew/0000-0001-9679-6020 FU U.S. Department of Energy, Office of Science, Early Career Research Program [DE-AC52-06NA25396] FX A.J.G. and M.B.J. thank the U.S. Department of Energy, Office of Science, Early Career Research Program (contract DE-AC52-06NA25396) for the experimental aspects of this work. In addition, an initial sample of the uranium complex 8 was prepared under the Heavy Element Chemistry Program, Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy. N.K. thanks UCL for computing resources via the Research Computing "Legion" cluster and associated services. NR 68 TC 55 Z9 55 U1 4 U2 71 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2041-6520 J9 CHEM SCI JI Chem. Sci. PY 2013 VL 4 IS 3 BP 1189 EP 1203 DI 10.1039/c2sc21806b PG 15 WC Chemistry, Multidisciplinary SC Chemistry GA 083OR UT WOS:000314474900041 ER PT J AU Shen, J Ward, TZ Yin, LF AF Shen Jian Ward, T. Z. Yin, L. F. TI Emergent phenomena in manganites under spatial confinement SO CHINESE PHYSICS B LA English DT Review DE manganites; metal-insulator transition; electrical transport; electronic phase separation ID PHASE-SEPARATED MANGANITES; ELECTRONIC PHASE; THIN-FILMS; DEPOSITION; OXIDES; PERCOLATION; PHYSICS AB It is becoming increasingly clear that the exotic properties displayed by correlated electronic materials such as high-T-c superconductivity in cuprates, colossal magnetoresistance (CMR) in manganites, and heavy-fermion compounds are intimately related to the coexistence of competing nearly degenerate states which couple simultaneously active degrees of freedom-charge, lattice, orbital, and spin states. The striking phenomena associated with these materials are due in a large part to spatial electronic inhomogeneities, or electronic phase separation (EPS). In many of these hard materials, the functionality is a result of the soft electronic component that leads to self-organization. In this paper, we review our recent work on a novel spatial confinement technique that has led to some fascinating new discoveries about the role of EPS in manganites. Using lithographic techniques to confine manganite thin films to length scales of the EPS domains that reside within them, it is possible to simultaneously probe EPS domains with different electronic states. This method allows for a much more complete view of the phases residing in a material and gives vital information on phase formation, movement, and fluctuation. Pushing this trend to its limit, we propose to control the formation process of the EPS using external local fields, which include magnetic exchange field, strain field, and electric field. We term the ability to pattern EPS "electronic nanofabrication." This method allows us to control the global physical properties of the system at a very fundamental level, and greatly enhances the potential for realizing true oxide electronics. C1 [Shen Jian; Yin, L. F.] Fudan Univ, State Key Lab Surface Phys, Shanghai 200433, Peoples R China. [Shen Jian; Yin, L. F.] Fudan Univ, Dept Phys, Shanghai 200433, Peoples R China. [Shen Jian] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Ward, T. Z.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Shen, J (reprint author), Fudan Univ, State Key Lab Surface Phys, Shanghai 200433, Peoples R China. EM shenj5494@fudan.edu.cn RI Ward, Thomas/I-6636-2016 OI Ward, Thomas/0000-0002-1027-9186 FU National Basic Research Program of China [2011CB921801]; National Natural Science Foundation of China [91121002, 11274071]; US DOE Office of Basic Energy Sciences, Scientific User Facilities Division; US DOE, US DOE Office of Basic Energy Sciences, Materials Sciences and Engineering Division, through the Oak Ridge National Laboratory [DE-SC0002136] FX Project supported by the National Basic Research Program of China (Grant No. 2011CB921801), the National Natural Science Foundation of China (Grant Nos. 91121002 and 11274071), US DOE Office of Basic Energy Sciences, Scientific User Facilities Division, and the US DOE grant DE-SC0002136, the US DOE Office of Basic Energy Sciences, Materials Sciences and Engineering Division, through the Oak Ridge National Laboratory. NR 41 TC 8 Z9 8 U1 6 U2 42 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1674-1056 J9 CHINESE PHYS B JI Chin. Phys. B PD JAN PY 2013 VL 22 IS 1 AR 017501 DI 10.1088/1674-1056/22/1/017501 PG 11 WC Physics, Multidisciplinary SC Physics GA 088DY UT WOS:000314815200087 ER PT J AU Wardle, KE Lee, T AF Wardle, Kent E. Lee, Taehun TI Finite element lattice Boltzmann simulations of free surface flow in a concentric cylinder SO COMPUTERS & MATHEMATICS WITH APPLICATIONS LA English DT Article; Proceedings Paper CT 7th International Conference for Mesoscopic Methods in Engineering and Science (ICMMES) CY JUL 12-16, 2010 CL Univ Alberta, Edmonton, CANADA HO Univ Alberta DE Finite element method; Lattice Boltzmann method; Free surface flow; Concentric cylinder ID ANNULAR CENTRIFUGAL CONTACTOR; EQUATION AB The annular centrifugal contactor is a compact mixer/centrifuge device designed for liquid-liquid extraction operations in processes for recycling nuclear fuel. The flow in the annulus of a centrifugal contactor is similar to the Taylor vortex flow with superimposed axial flow. The major differences are that the contactor has one end that is open to air and the free surface effects dominate the annular flow. In this study, we demonstrate the application of a finite element lattice Boltzmann equation (FE-LBE) method to the annular mixing geometry as found in a centrifugal contactor. The computational results are validated with available experimental observations with the Reynolds number (Re) in the range of 1250 < Re < 2000. The rotation rate of the inner cylinder determines the final flow modes, and time-dependent traveling waves emerge past a critical Re. (C) 2011 Elsevier Ltd. All rights reserved. C1 [Wardle, Kent E.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Lee, Taehun] CUNY City Coll, Dept Mech Engn, New York, NY 10031 USA. RP Lee, T (reprint author), CUNY City Coll, Dept Mech Engn, New York, NY 10031 USA. EM kwardle@anl.gov; thlee@ccny.cuny.edu RI Lee, Taehun/G-2695-2010 OI Lee, Taehun/0000-0001-9965-5637 NR 18 TC 5 Z9 5 U1 0 U2 22 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0898-1221 EI 1873-7668 J9 COMPUT MATH APPL JI Comput. Math. Appl. PD JAN PY 2013 VL 65 IS 2 SI SI BP 230 EP 238 DI 10.1016/j.camwa.2011.09.020 PG 9 WC Mathematics, Applied SC Mathematics GA 078BM UT WOS:000314073100009 ER PT J AU Uga, KC Min, MS Lee, T Fischer, PF AF Uga, Kalu Chibueze Min, Misun Lee, Taehun Fischer, Paul F. TI Spectral-element discontinuous Galerkin lattice Boltzmann simulation of flow past two cylinders in tandem with an exponential time integrator SO COMPUTERS & MATHEMATICS WITH APPLICATIONS LA English DT Article; Proceedings Paper CT 7th International Conference for Mesoscopic Methods in Engineering and Science (ICMMES) CY JUL 12-16, 2010 CL Univ Alberta, Edmonton, CANADA HO Univ Alberta DE Lattice Boltzmann method; Exponential integrator; Spectral element; Discontinuous Galerkin; Tandem cylinders ID CIRCULAR-CYLINDER; NUMERICAL-SOLUTIONS; REYNOLDS-NUMBERS; EQUATION; MODEL AB In this paper, a spectral-element discontinuous Galerkin (SEDG) lattice Boltzmann discretization and an exponential time-marching scheme are used to study the flow field past two circular cylinders in tandem arrangement. The basic idea is to discretize the streaming step of the lattice Boltzmann equation by using the SEDG method to get a system of ordinary differential equations (ODEs) whose exact solutions are expressed by using a large matrix exponential. The approximate solution of the resulting ODEs are obtained from a projection method based on a Krylov subspace approximation. This approach allows us to approximate the matrix exponential of a very large and sparse matrix by using a matrix of much smaller dimension. The exponential time integration scheme is useful especially when computations are carried out at high Courant-Friedrichs-Lewy (CFL) numbers, where most explicit time-marching schemes are inaccurate. Simulations of flow were carried out for a circular cylinder at Re = 20 and for two circular cylinders in tandem at Re = 40 and a spacing of 2.5D, where D is the diameter of the cylinders. We compare our results with those from a fourth-order Runge-Kutta scheme that is restricted by the CFL number. In addition, important flow parameters such as the drag coefficients of the two cylinders and the wake length behind the rear cylinder were calculated by using the exponential time integration scheme. These results are compared with results from our simulation using the RK scheme and with existing benchmark results. (C) 2012 Elsevier Ltd. All rights reserved. C1 [Uga, Kalu Chibueze; Lee, Taehun] CUNY City Coll, Dept Mech Engn, New York, NY 10031 USA. [Min, Misun; Fischer, Paul F.] Argonne Natl Lab, Div Math & Comp Sci, Argonne, IL 60439 USA. RP Lee, T (reprint author), CUNY City Coll, Dept Mech Engn, New York, NY 10031 USA. EM kuga00@ccny.cuny.edu; mmin@mcs.anl.gov; thlee@ccny.cuny.edu; fischer@mcs.anl.gov RI Lee, Taehun/G-2695-2010 OI Lee, Taehun/0000-0001-9965-5637 NR 31 TC 4 Z9 4 U1 0 U2 13 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0898-1221 J9 COMPUT MATH APPL JI Comput. Math. Appl. PD JAN PY 2013 VL 65 IS 2 SI SI BP 239 EP 251 DI 10.1016/j.camwa.2011.12.059 PG 13 WC Mathematics, Applied SC Mathematics GA 078BM UT WOS:000314073100010 ER EF