FN Thomson Reuters Web of Science™ VR 1.0 PT J AU Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hammer, J Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Liko, D Mikulec, I Pernicka, M Rahbaran, B Rohringer, C Rohringer, H Schofbeck, R Strauss, J Taurok, A Wagner, P Waltenberger, W Walzel, G Widl, E Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Bansal, S Cornelis, T De Wolf, EA Janssen, X Luyckx, S Maes, T Mucibello, L Ochesanu, S Roland, B Rougny, R Selvaggi, M Staykova, Z Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Suarez, RG Kalogeropoulos, A Maes, M Olbrechts, A Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Charaf, O Clerbaux, B De Lentdecker, G Dero, V Gay, APR Hreus, T Leonard, A Marage, PE Reis, T Thomas, L Vander Velde, C Vanlaer, P Wang, J Adler, V Beernaert, K Cimmino, A Costantini, S Garcia, G Grunewald, M Klein, B Lellouch, J Marinov, A Mccartin, J Rios, AAO Ryckbosch, D Strobbe, N Thyssen, F Tytgat, M Vanelderen, L Verwilligen, P Walsh, S Yazgan, E Zaganidis, N Basegmez, S Bruno, G Castello, R Caudron, A Ceard, L Delaere, C du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Lemaitre, V Liao, J Militaru, O Nuttens, C Pagano, D Perrini, L Pin, A Piotrzkowski, K Schul, N Garcia, JMV Beliy, N Caebergs, T Daubie, E Hammad, GH Alves, GA Martins, MC Damiao, DD Martins, T Pol, ME Souza, MHG Alda, WL Carvalho, W Custodio, A Da Costa, EM Martins, CD De Souza, SF Figueiredo, DM Mundim, L Nogima, H Oguri, V Da Silva, WLP Santoro, A Jorge, LS Sznajder, A Bernardes, CA Dias, FA Tomei, TRFP Gregores, EM Lagana, C Marinho, F Mercadante, PG Novaes, SF Padula, SS Genchev, V Iaydjiev, P Piperov, S Rodozov, M Stoykova, S Sultanov, G Tcholakov, V Trayanov, R Vutova, M Dimitrov, A Hadjiiska, R Kozhuharov, V Litov, L Pavlov, B Petkov, P Bian, JG Chen, GM Chen, HS Jiang, CH Liang, D Liang, 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Chung, Y. S. Covarelli, R. de Barbaro, P. Demina, R. Eshaq, Y. Garcia-Bellido, A. Goldenzweig, P. Han, J. Harel, A. Miner, D. C. Vishnevskiy, D. Zielinski, M. Bhatti, A. Ciesielski, R. Demortier, L. Goulianos, K. Lungu, G. Malik, S. Mesropian, C. Arora, S. Barker, A. Chou, J. P. Contreras-Campana, C. Contreras-Campana, E. Duggan, D. Ferencek, D. Gershtein, Y. Gray, R. Halkiadakis, E. Hidas, D. Lath, A. Panwalkar, S. Park, M. Patel, R. Rekovic, V. Robles, J. Rose, K. Salur, S. Schnetzer, S. Seitz, C. Somalwar, S. Stone, R. Thomas, S. Cerizza, G. Hollingsworth, M. Spanier, S. Yang, Z. C. York, A. Eusebi, R. Flanagan, W. Gilmore, J. Kamon, T. Khotilovich, V. Montalvo, R. Osipenkov, I. Pakhotin, Y. Perloff, A. Roe, J. Safonov, A. Sakuma, T. Sengupta, S. Suarez, I. Tatarinov, A. Toback, D. Akchurin, N. Damgov, J. Dudero, P. R. Jeong, C. Kovitanggoon, K. Lee, S. W. Libeiro, T. Roh, Y. Volobouev, I. Appelt, E. Florez, C. Greene, S. Gurrola, A. Johns, W. Johnston, C. Kurt, P. Maguire, C. Melo, A. Sheldon, P. Snook, B. Tuo, S. Velkovska, J. Arenton, M. W. Balazs, M. Boutle, S. Cox, B. Francis, B. Goodell, J. Hirosky, R. Ledovskoy, A. Lin, C. Neu, C. Wood, J. Yohay, R. Gollapinni, S. Harr, R. Karchin, P. E. Don, C. Kottachchi Kankanamge Lamichhane, P. Sakharov, A. Anderson, M. Bachtis, M. Belknap, D. Borrello, L. Carlsmith, D. Cepeda, M. Dasu, S. Gray, L. Grogg, K. S. Grothe, M. Hall-Wilton, R. Herndon, M. Herve, A. Klabbers, P. Klukas, J. Lanaro, A. Lazaridis, C. Leonard, J. Loveless, R. Mohapatra, A. Ojalvo, I. Palmonari, F. Pierro, G. A. Ross, I. Savin, A. Smith, W. H. Swanson, J. CA CMS Collaboration TI A search for a doubly-charged Higgs boson in pp collisions at root s=7 TeV SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID NEUTRINO MASSES; BHABHA SCATTERING; VIOLATION; MODELS; DECAY; LHC; LEP AB A search for a doubly-charged Higgs boson in pp collisions at root s = 7 TeV is presented. The data correspond to an integrated luminosity of 4.9 fb(-1), collected by the CMS experiment at the LHC. The search is performed using events with three or more isolated charged leptons of any flavor, giving sensitivity to the decays of pair-produced triplet components Phi(++)Phi(--), and Phi(++)Phi(-) from associated production. No excess is observed compared to the background prediction, and upper limits at the 95 % confidence level are set on the Phi(++) production cross section, under specific assumptions on its branching fractions. Lower bounds on the Phi(++) mass are reported, providing significantly more stringent constraints than previously published limits. C1 [Chatrchyan, S.; Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Bergauer, T.; Dragicevic, M.; Eroe, J.; Fabjan, C.; Friedl, M.; Fruehwirth, R.; Ghete, V. 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M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Meneghelli, M.; Montanari, A.; Navarria, F. L.; Odorici, F.; Perrotta, A.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G.; Travaglini, R.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Capiluppi, P.; Castro, A.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Meneghelli, M.; Navarria, F. L.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gallo, E.; Gonzi, S.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gonzi, S.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Colafranceschi, S.; Fabbri, F.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Fabbricatore, P.; Musenich, R.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Benaglia, A.; De Guio, F.; Di Matteo, L.; Fiorendi, S.; Gennai, S.; Ghezzi, A.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Massironi, A.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; Sala, S.; de Fatis, T. Tabarelli] Ist Nazl Fis Nucl, Sez Milano Bicocca, I-20133 Milan, Italy. [Benaglia, A.; De Guio, F.; Di Matteo, L.; Fiorendi, S.; Ghezzi, A.; Manzoni, R. A.; Martelli, A.; Massironi, A.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Montoya, C. A. Carrillo; Cavallo, N.; De Cosa, A.; Dogangun, O.; Fabozzi, F.; Iorio, A. O. M.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [De Cosa, A.; Dogangun, O.; Merola, M.] Univ Naples Federico II, Naples, Italy. [Azzi, P.; Bacchetta, N.; Bisello, D.; Branca, A.; Carlin, R.; Checchia, P.; Dorigo, T.; Dosselli, U.; Gasparini, F.; Gasparini, U.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Lazzizzera, I.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Vanini, S.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Bisello, D.; Carlin, R.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Vanini, S.; Zotto, P.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.; Lazzizzera, I.] Univ Trento Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Torre, P.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Torre, P.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Fano, L.; Lariccia, P.; Lucaroni, A.; Mantovani, G.; Menichelli, M.; Nappi, A.; Romeo, F.; Saha, A.; Santocchia, A.; Taroni, S.; Pioppi, M.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Biasini, M.; Fano, L.; Lariccia, P.; Lucaroni, A.; Mantovani, G.; Nappi, A.; Romeo, F.; Santocchia, A.; Taroni, S.; Pioppi, M.] Univ Perugia, I-06100 Perugia, Italy. [Azzurri, P.; Bagliesi, G.; Boccali, T.; Broccolo, G.; Castaldi, R.; D'Agnolo, R. T.; Dell'Orso, R.; Fiori, F.; Foa, L.; Giassi, A.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Fiori, F.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Azzurri, P.; Broccolo, G.; D'Agnolo, R. T.; Foa, L.; Ligabue, F.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Diemoz, M.; Grassi, M.; Longo, E.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Sigamani, M.; Soffi, L.; Rovelli, C.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; Del Re, D.; Grassi, M.; Longo, E.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Soffi, L.; Rovelli, C.] Univ Roma La Sapienza, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Biino, C.; Cartiglia, N.; Costa, M.; Demaria, N.; Graziano, A.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Pastrone, N.; Pelliccioni, M.; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Sola, V.; Solano, A.; Staiano, A.; Pereira, A. Vilela] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Costa, M.; Graziano, A.; Migliore, E.; Monaco, V.; Potenza, A.; Romero, A.; Sacchi, R.; Sola, V.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; Marone, M.; Montanino, D.; Penzo, A.; Schizzi, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; Marone, M.; Montanino, D.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Heo, S. G.; Kim, T. Y.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Chang, S.; Chung, J.; Kim, D. H.; Kim, G. N.; Kong, D. J.; Park, H.; Ro, S. R.; Son, D. C.; Son, T.; Kamon, T.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, J. Y.; Kim, Z. J.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, T. J.; Lee, K. S.; Moon, D. H.; Park, S. K.] Korea Univ, Seoul, South Korea. [Choi, M.; Kang, S.; Kim, J. H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Cho, Y.; Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. S.; Kwon, E.; Lee, B.; Lee, J.; Lee, S.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Bilinskas, M. J.; Grigelionis, I.; Janulis, M.; Juodagalvis, A.] Vilnius Univ, Vilnius, Lithuania. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Lopez-Fernandez, R.; Magana Villalba, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.; Reyes-Santos, M. A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Bell, A. J.; Butler, P. H.; Doesburg, R.; Reucroft, S.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Asghar, M. I.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bluj, M.; Bialkowska, H.; Boimska, B.; Frueboes, T.; Gokieli, R.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Soltan Inst Nucl Studies, PL-00681 Warsaw, Poland. [Almeida, N.; Bargassa, P.; David, A.; Faccioli, P.; Fernandes, M.; Ferreira Parracho, P. G.; Gallinaro, M.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Belotelov, I.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Kozlov, G.; Lanev, A.; Malakhov, A.; Moisenz, P.; Palichik, V.; Perelygin, V.; Savina, M.; Shmatov, S.; Smirnov, V.; Volodko, A.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Evstyukhin, S.; Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Matveev, V.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow, Russia. [Epshteyn, V.; Erofeeva, M.; Gavrilov, V.; Kossov, M.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Stolin, V.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Zhukov, V.; Katkov, I.; Belyaev, A.; Boos, E.; Bunichev, V.; Dubinin, M.; Dudko, L.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Markina, A.; Obraztsov, S.; Perfilov, M.; Petrushanko, S.; Popov, A.; Sarycheva, L.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Grishin, V.; Kachanov, V.; Konstantinov, D.; Korablev, A.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Alcaraz Maestre, J.; Arce, P.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Diez Pardos, C.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.; Willmott, C.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain. [Albajar, C.; Codispoti, G.; de Troconiz, J. F.] Univ Autonoma Madrid, Madrid, Spain. [Fernandes, M.; Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Chuang, S. H.; Duarte Campderros, J.; Felcini, M.; Gomez, G.; Gonzalez Sanchez, J.; Jorda, C.; Lobelle Pardo, P.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Sobron Sanudo, M.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, Inst Fis Cantabria IFCA, CSIC, E-39005 Santander, Spain. [Genchev, V.; Iaydjiev, P.; Puljak, I.; Chierici, R.; Guthoff, M.; Hauth, T.; Foudas, C.; Hajdu, C.; Sharma, A.; Mohanty, A. 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Gomez-Reino; Govoni, P.; Gowdy, S.; Guida, R.; Hansen, M.; Harris, P.; Hartl, C.; Harvey, J.; Hegner, B.; Hinzmann, A.; Innocente, V.; Janot, P.; Kaadze, K.; Karavakis, E.; Kousouris, K.; Lecoq, P.; Lee, Y-J.; Lenzi, P.; Lourenco, C.; Maeki, T.; Malberti, M.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moser, R.; Mozer, M. U.; Mulders, M.; Musella, P.; Nesvold, E.; Orimoto, T.; Orsini, L.; Cortezon, E. Palencia; Perez, E.; Perrozzi, L.; Petrilli, A.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Piparo, D.; Polese, G.; Quertenmont, L.; Racz, A.; Reece, W.; Antunes, J. Rodrigues; Rolandi, G.; Rommerskirchen, T.; Rovelli, C.; Rovere, M.; Sakulin, H.; Santanastasio, F.; Schaefer, C.; Schwick, C.; Segoni, I.; Sekmen, S.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Spiropulu, M.; Stoye, M.; Tsirou, A.; Veres, G. I.; Vlimant, J. R.; Woehri, H. K.; Worm, S. D.; Zeuner, W. D.; Pela, J.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Gabathuler, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Meier, F.; Renker, D.; Rohe, T.; Sibille, J.; Naegeli, C.] Paul Scherrer Inst, Villigen, Switzerland. [Baeni, L.; Bortignon, P.; Buchmann, M. A.; Casal, B.; Chanon, N.; Deisher, A.; Dissertori, G.; Dittmar, M.; Duenser, M.; Eugster, J.; Freudenreich, K.; Grab, C.; Hits, D.; Lecomte, P.; Lustermann, W.; Marini, A. C.; del Arbol, P. Martinez Ruiz; Mohr, N.; Moortgat, F.; Naegeli, C.; Nef, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pape, L.; Pauss, F.; Peruzzi, M.; Ronga, F. J.; Rossini, M.; Sala, L.; Sanchez, A. K.; Starodumov, A.; Stieger, B.; Takahashi, M.; Tauscher, L.; Thea, A.; Theofilatos, K.; Treille, D.; Urscheler, C.; Wallny, R.; Weber, H. A.; Wehrli, L.] ETH, Inst Particle Phys, Zurich, Switzerland. [Aguilo, E.; Amsler, C.; Chiochia, V.; De Visscher, S.; Favaro, C.; Rikova, M. Ivova; Mejias, B. Millan; Otiougova, P.; Robmann, P.; Snoek, H.; Tupputi, S.; Verzetti, M.] Univ Zurich, Zurich, Switzerland. [Chang, Y. H.; Chen, K. H.; Kuo, C. M.; Li, S. W.; Lin, W.; Liu, Z. K.; Lu, Y. J.; Mekterovic, D.; Singh, A. P.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Wang, X.; Chang, Y. H.; Bartalini, P.; Chang, P.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Dietz, C.; Grundler, U.; Hou, W-S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Lu, R-S.; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wang, M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Karapinar, G.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, L. N.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Yildirim, E.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey. [Cankocak, K.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.] Natl Sci Ctr, Kharkov Inst Phys & Technol, Kharkov, Ukraine. [Bostock, F.; Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Kreczko, L.; Metson, S.; Newbold, D. M.; Nirunpong, K.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Worm, S. D.; Newbold, D. M.; Basso, L.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Jackson, J.; Kennedy, B. W.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Womersley, W. J.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Bainbridge, R.; Ball, G.; Beuselinck, R.; Buchmuller, O.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Lyons, L.; Magnan, A-M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Papageorgiou, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Ryan, M. J.; Seez, C.; Sharp, P.; Sparrow, A.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.; Whyntie, T.] Univ London Imperial Coll Sci Technol & Med, London, England. [Chadwick, M.; Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Hatakeyama, K.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; St John, J.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Bhattacharya, S.; Alimena, J.; Cutts, D.; Ferapontov, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Nguyen, D.; Segala, M.; Sinthuprasith, T.; Speer, T.; Tsang, K. V.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Dolen, J.; Erbacher, R.; Gardner, M.; Houtz, R.; Ko, W.; Kopecky, A.; Lander, R.; Miceli, T.; Pellett, D.; Rutherford, B.; Searle, M.; Smith, J.; Squires, M.; Tripathi, M.; Sierra, R. Vasquez] Univ Calif Davis, Davis, CA 95616 USA. [Andreev, V.; Felcini, M.; Cline, D.; Cousins, R.; Duris, J.; Erhan, S.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Plager, C.; Rakness, G.; Schlein, P.; Tucker, J.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Liu, H.; Babb, J.; Clare, R.; Dinardo, M. E.; Ellison, J.; Gary, J. W.; Giordano, F.; Hanson, G.; Jeng, G. Y.; Long, O. R.; Luthra, A.; Nguyen, H.; Paramesvaran, S.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sharma, V.; Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; Evans, D.; Golf, F.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Macneill, I.; Mangano, B.; Padhi, S.; Palmer, C.; Petrucciani, G.; Pieri, M.; Sani, M.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bellan, R.; Campagnari, C.; D'Alfonso, M.; Danielson, T.; Flowers, K.; Geffert, P.; Incandela, J.; Justus, C.; Kalavase, P.; Koay, S. A.; Kovalskyi, D.; Krutelyov, V.; Lowette, S.; Mccoll, N.; Pavlunin, V.; Rebassoo, F.; Ribnik, J.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dias, F. A.; Dubinin, M.; Spiropulu, M.; Apresyan, A.; Bornheim, A.; Chen, Y.; Di Marco, E.; Duarte, J.; Gataullin, M.; Ma, Y.; Mott, A.; Newman, H. B.; Rogan, C.; Timciuc, V.; Traczyk, P.; Veverka, J.; Wilkinson, R.; Yang, Y.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Akgun, B.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Liu, Y. F.; Paulini, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Edelmaier, C. J.; Ford, W. T.; Gaz, A.; Heyburn, B.; Lopez, E. Luiggi; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Eggert, N.; Gibbons, L. K.; Heltsley, B.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Vaughan, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bloch, I.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Green, D.; Gutsche, O.; Hanlon, J.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Kilminster, B.; Klima, B.; Kunori, S.; Kwan, S.; Leonidopoulos, C.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Tan, P.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Wu, W.; Yang, F.; Yumiceva, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Piedra Gomez, J.; Acosta, D.; Avery, P.; Bourilkov, D.; Chen, M.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Drozdetskiy, A.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Gartner, J.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Remington, R.; Rinkevicius, A.; Sellers, P.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Lebolo, L. M.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, J. R.; Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Gleyzer, S. V.; Haas, J.; Hagopian, S.; Hagopian, V.; Jenkins, M.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Vodopiyanov, I.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Anghel, I. M.; Apanasevich, L.; Bai, Y.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Callner, J.; Cavanaugh, R.; Dragoiu, C.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Lacroix, F.; Malek, M.; O'Brien, C.; Silkworth, C.; Strom, D.; Varelas, N.] UIC, Chicago, IL USA. [Ozturk, S.; Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Duru, F.; Griffiths, S.; Merlo, J-P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Newsom, C. R.; Norbeck, E.; Onel, Y.; Ozok, F.; Sen, S.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Giurgiu, G.; Gritsan, A. V.; Guo, Z. J.; Hu, G.; Maksimovic, P.; Rappoccio, S.; Swartz, M.; Whitbeck, A.] Johns Hopkins Univ, Baltimore, MD USA. [Sibille, J.; Baringer, P.; Bean, A.; Benelli, G.; Grachov, O.; Kenny, R. P., III; Murray, M.; Noonan, D.; Sanders, S.; Stringer, R.; Tinti, G.; Wood, J. S.; Zhukova, V.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Bolton, T.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Boutemeur, M.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kirn, M.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Peterman, A.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.; Twedt, E.] Univ Maryland, College Pk, MD 20742 USA. [Li, W.; Bauer, G.; Bendavid, J.; Busza, W.; Butz, E.; Cali, I. A.; Chan, M.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Hahn, K. A.; Kim, Y.; Klute, M.; Krajczar, K.; Luckey, P. D.; Ma, T.; Nahn, S.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Rudolph, M.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Sung, K.; Velicanu, D.; Wenger, E. A.; Wolf, R.; Wyslouch, B.; Xie, S.; Yang, M.; Yilmaz, Y.; Yoon, A. S.; Zanetti, M.] MIT, Cambridge, MA 02139 USA. [Cooper, S. I.; Dahmes, B.; De Benedetti, A.; Franzoni, G.; Gude, A.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Sasseville, M.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Cremaldi, L. M.; Kroeger, R.; Perera, L.; Rahmat, R.; Sanders, D. A.] Univ Mississippi, University, MS 38677 USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Butt, J.; Claes, D. R.; Dominguez, A.; Eads, M.; Keller, J.; Kravchenko, I.; Lazo-Flores, J.; Malbouisson, H.; Malik, S.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Baur, U.; Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Shipkowski, S. P.; Smith, K.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Nash, D.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Anastassov, A.; Kubik, A.; Mucia, N.; Odell, N.; Ofierzynski, R. A.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Velasco, M.; Won, S.] Northeastern Univ, Evanston, IL USA. [Antonelli, L.; Berry, D.; Brinkerhoff, A.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kolb, J.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Morse, D. M.; Pearson, T.; Ruchti, R.; Slaunwhite, J.; Valls, N.; Wayne, M.; Wolf, M.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Bylsma, B.; Durkin, L. S.; Hart, A.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Puigh, D.; Rodenburg, M.; Vuosalo, C.; Williams, G.; Winer, B. L.] Ohio State Univ, Columbus, OH 43210 USA. [Adam, N.; Berry, E.; Elmer, P.; Gerbaudo, D.; Halyo, V.; Hebda, P.; Hegeman, J.; Hunt, A.; Jindal, P.; Pegna, D. Lopes; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Raval, A.; Safdi, B.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Acosta, J. G.; Brownson, E.; Huang, X. T.; Lopez, A.; Mendez, H.; Oliveros, S.; Vargas, J. E. Ramirez; Zatserklyaniy, A.] Univ Puerto Rico, Mayaguez, PR USA. [Alagoz, E.; Barnes, V. E.; Benedetti, D.; Bolla, G.; Bortoletto, D.; De Mattia, M.; Everett, A.; Hu, Z.; Jones, M.; Koybasi, O.; Kress, M.; Laasanen, A. T.; Leonardo, N.; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Marono, M. Vidal; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Guragain, S.; Parashar, N.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Boulahouache, C.; Ecklund, K. M.; Geurts, F. J. M.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; Chung, Y. S.; Covarelli, R.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Miner, D. C.; Vishnevskiy, D.; Zielinski, M.] Univ Rochester, Rochester, NY 14627 USA. [Malik, S.; Bhatti, A.; Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Lath, A.; Panwalkar, S.; Park, M.; Patel, R.; Rekovic, V.; Robles, J.; Rose, K.; Salur, S.; Schnetzer, S.; Seitz, C.; Somalwar, S.; Stone, R.; Thomas, S.] Rutgers State Univ, Piscataway, NJ USA. [Cerizza, G.; Hollingsworth, M.; Spanier, S.; Yang, Z. C.; York, A.] Univ Tennessee, Knoxville, TN USA. [Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Khotilovich, V.; Montalvo, R.; Osipenkov, I.; Pakhotin, Y.; Perloff, A.; Roe, J.; Safonov, A.; Sakuma, T.; Sengupta, S.; Suarez, I.; Tatarinov, A.; Toback, D.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Damgov, J.; Dudero, P. R.; Jeong, C.; Kovitanggoon, K.; Lee, S. W.; Libeiro, T.; Roh, Y.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Appelt, E.; Florez, C.; Greene, S.; Gurrola, A.; Johns, W.; Johnston, C.; Kurt, P.; Maguire, C.; Melo, A.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN USA. [Arenton, M. W.; Balazs, M.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Lin, C.; Neu, C.; Wood, J.; Yohay, R.] Univ Virginia, Charlottesville, VA USA. [Gollapinni, S.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sakharov, A.] Wayne State Univ, Detroit, MI USA. [Anderson, M.; Bachtis, M.; Belknap, D.; Borrello, L.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Gray, L.; Grogg, K. S.; Grothe, M.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Klukas, J.; Lanaro, A.; Lazaridis, C.; Leonard, J.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Palmonari, F.; Pierro, G. A.; Ross, I.; Savin, A.; Smith, W. H.; Swanson, J.] Univ Wisconsin, Madison, WI 53706 USA. 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[Colafranceschi, S.] Univ Rome, Fac Ingn, Rome, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata, I-85100 Potenza, Italy. [Meola, S.] Univ Guglielmo Marconi, Rome, Italy. [Martini, L.] Univ Siena, I-53100 Siena, Italy. [Serban, A. T.] Univ Bucharest, Fac Phys, Bucharest, Romania. [Rolandi, G.] Ist Nazl Fis Nucl, Scuola Normale, Pisa, Italy. [Bakirci, M. N.; Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey. [Cerci, S.; Cerci, D. Sunar; Tali, B.] Adiyaman Univ, Adiyaman, Turkey. [Sogut, K.] Mersin Univ, Mersin, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Kaya, M.; Kaya, O.] Kafkas Univ, Kars, Turkey. [Ozkorucuklu, S.] Suleyman Demirel Univ, TR-32200 Isparta, Turkey. [Sonmez, N.] Ege Univ, Izmir, Turkey. [Basso, L.; Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Jeng, G. Y.] Univ Sydney, Sydney, NSW 2006, Australia. [Wasserbaech, S.] Utah Valley Univ, Orem, UT USA. [Bilki, B.] Argonne Natl Lab, Argonne, IL 60439 USA. 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Dogangun, Oktay/0000-0002-1255-2211; Martelli, Arabella/0000-0003-3530-2255; Gonzi, Sandro/0000-0003-4754-645X; Levchenko, Petr/0000-0003-4913-0538; Varela, Joao/0000-0003-2613-3146; Heath, Helen/0000-0001-6576-9740; Sguazzoni, Giacomo/0000-0002-0791-3350; Ligabue, Franco/0000-0002-1549-7107; Diemoz, Marcella/0000-0002-3810-8530; Tricomi, Alessia Rita/0000-0002-5071-5501; Fassi, Farida/0000-0002-6423-7213; Heredia De La Cruz, Ivan/0000-0002-8133-6467; Ghezzi, Alessio/0000-0002-8184-7953; bianco, stefano/0000-0002-8300-4124; Demaria, Natale/0000-0003-0743-9465; Benaglia, Andrea Davide/0000-0003-1124-8450; Covarelli, Roberto/0000-0003-1216-5235; Ciulli, Vitaliano/0000-0003-1947-3396; Fiorendi, Sara/0000-0003-3273-9419; Bean, Alice/0000-0001-5967-8674; Longo, Egidio/0000-0001-6238-6787; Di Matteo, Leonardo/0000-0001-6698-1735; Baarmand, Marc/0000-0002-9792-8619; Boccali, Tommaso/0000-0002-9930-9299; Menasce, Dario Livio/0000-0002-9918-1686; Bargassa, Pedrame/0000-0001-8612-3332; Attia Mahmoud, Mohammed/0000-0001-8692-5458; Bilki, Burak/0000-0001-9515-3306; Safdi, Benjamin R./0000-0001-9531-1319; Lloret Iglesias, Lara/0000-0002-0157-4765; Haj Ahmad, Wael/0000-0003-1491-0446; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Gerbaudo, Davide/0000-0002-4463-0878; Vieira de Castro Ferreira da Silva, Pedro Manuel/0000-0002-5725-041X; Hernandez Calama, Jose Maria/0000-0001-6436-7547; TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; Arce, Pedro/0000-0003-3009-0484; Flix, Josep/0000-0003-2688-8047; Della Ricca, Giuseppe/0000-0003-2831-6982; Paganoni, Marco/0000-0003-2461-275X; Gulmez, Erhan/0000-0002-6353-518X; Seixas, Joao/0000-0002-7531-0842; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; D'Alessandro, Raffaello/0000-0001-7997-0306; Belyaev, Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279; Konecki, Marcin/0000-0001-9482-4841; Bedoya, Cristina/0000-0001-8057-9152; Matorras, Francisco/0000-0003-4295-5668; My, Salvatore/0000-0002-9938-2680; Rovelli, Tiziano/0000-0002-9746-4842; Calvo Alamillo, Enrique/0000-0002-1100-2963; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Marinho, Franciole/0000-0002-7327-0349; Ferguson, Thomas/0000-0001-5822-3731; Ragazzi, Stefano/0000-0001-8219-2074; Benussi, Luigi/0000-0002-2363-8889; Grandi, Claudio/0000-0001-5998-3070; Lazzizzera, Ignazio/0000-0001-5092-7531; Sen, Sercan/0000-0001-7325-1087; de Jesus Damiao, Dilson/0000-0002-3769-1680; Codispoti, Giuseppe/0000-0003-0217-7021; Cerrada, Marcos/0000-0003-0112-1691; Azzi, Patrizia/0000-0002-3129-828X; Scodellaro, Luca/0000-0002-4974-8330; FU FMSR (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MES (Bulgaria); CERN; CAS (China); MoST (China); NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); MoER [SF0690030s09]; ERDF (Estonia); Academy of Finland (Finland); MEC (Finland); HIP (Finland); CEA (France); CNRS/IN2P3 (France); BMBF (Germany); DFG (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NKTH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF (Korea); WCU (Korea); LAS (Lithuania); CINVESTAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); MSI (New Zealand); PAEC (Pakistan); MSHE (Poland); NSC (Poland); FCT (Portugal); JINR (Armenia); JINR (Belarus); JINR (Georgia); JINR (Ukraine); JINR (Uzbekistan); MON (Russia); RosAtom (Russia); RAS (Russia); RFBR (Russia); MSTD (Serbia); MICINN (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); TUBITAK (Turkey); STFC (United Kingdom); DOE (USA); NSF (USA); Marie-Curie programme; European Research Council (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Council of Science and Industrial Research, India; HOMING PLUS programme of Foundation for Polish Science; European Union, Regional Development Fund FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC machine. We thank the technical and administrative staff at CERN and other CMS institutes, and acknowledge support from: FMSR (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); MoER, SF0690030s09 and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NKTH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF and WCU (Korea); LAS (Lithuania); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MSI (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Armenia, Belarus, Georgia, Ukraine, Uzbekistan); MON, RosAtom, RAS and RFBR (Russia); MSTD (Serbia); MICINN and CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); TUBITAK and TAEK (Turkey); STFC (United Kingdom); DOE and NSF (USA). Individuals have received support from the Marie-Curie programme and the European Research Council (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Council of Science and Industrial Research, India; and the HOMING PLUS programme of Foundation for Polish Science, co-financed from European Union, Regional Development Fund. NR 55 TC 64 Z9 64 U1 1 U2 75 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD NOV PY 2012 VL 72 IS 11 AR 2189 DI 10.1140/epjc/s10052-012-2189-5 PG 26 WC Physics, Particles & Fields SC Physics GA 050SR UT WOS:000312074800002 ER PT J AU Johnson, TC Versteeg, RJ Rockhold, M Slater, LD Ntarlagiannis, D Greenwood, WJ Zachara, J AF Johnson, Timothy C. Versteeg, Roelof J. Rockhold, Mark Slater, Lee D. Ntarlagiannis, Dimitrios Greenwood, William J. Zachara, John TI Characterization of a contaminated wellfield using 3D electrical resistivity tomography implemented with geostatistical, discontinuous boundary, and known conductivity constraints SO GEOPHYSICS LA English DT Article ID GROSS EARTH DATA; INDUCED-POLARIZATION; OCCAMS INVERSION; DC-RESISTIVITY; TRANSPORT; AQUIFER; MODEL; SITE; FLOW; SEDIMENTS AB Continuing advancements in subsurface electrical resistivity tomography (ERT) are increasing its capabilities for understanding shallow subsurface properties and processes. The inability of ERT imaging data to resolve unique subsurface structures and the corresponding need to include constraining information remains one of the greatest limitations, yet provides one of the greatest opportunities for further advancing the utility of the method. We propose a new method of incorporating constraining information into an ERT imaging algorithm in the form of discontinuous boundaries, known values, and spatial covariance information. We demonstrated the approach by imaging a uranium-contaminated wellfield at the Hanford Site in southeastern Washington State, USA. We incorporate into the algorithm known boundary information and spatial covariance structures derived from the highly resolved near-borehole regions of a regularized ERT inversion. The resulting inversion provides a solution which fits the ERT data (given the estimated noise level), honors the spatial covariance structure throughout the model, and is consistent with known bulk-conductivity discontinuities. The results are validated with core-scale measurements, indicating a significant improvement in accuracy over the standard regularized inversion and revealing important subsurface structure known to influence flow and transport at the site. C1 [Johnson, Timothy C.; Rockhold, Mark; Zachara, John] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. [Versteeg, Roelof J.] Subsurface Insights LLC, Hanover, NH USA. [Slater, Lee D.; Ntarlagiannis, Dimitrios] Rutgers State Univ, Dept Earth & Environm Sci, Newark, NJ 07102 USA. [Greenwood, William J.] Adv Geosci Inc, Austin, TX USA. RP Johnson, TC (reprint author), Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. EM tj@pnnl.gov; roelof.versteeg@subsurfaceinsights.com; mark.rockhold@pnnl.gov; lstater@andromeda.rutgers.edu; dimntar@andromeda.rutgers.edu; wjgreenwood@gmx.com; john.zachara@pnnl.gov FU Office of Biological and Environmental Research, U.S. Department of Energy, as part of the Hanford 300 Area Integrated Field Research Challenge project FX We appreciate the constructive reviews of this manuscript by Allain Plattner and two anonymous referees. This work was funded by the Office of Biological and Environmental Research, U.S. Department of Energy, as part of the Hanford 300 Area Integrated Field Research Challenge project. We gratefully acknowledge Andy Ward and Chris Strickland for facilitating field data collection efforts. NR 51 TC 9 Z9 9 U1 3 U2 22 PU SOC EXPLORATION GEOPHYSICISTS PI TULSA PA 8801 S YALE ST, TULSA, OK 74137 USA SN 0016-8033 EI 1942-2156 J9 GEOPHYSICS JI Geophysics PD NOV-DEC PY 2012 VL 77 IS 6 BP EN85 EP EN96 DI 10.1190/GEO2012-0121.1 PG 12 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA 061CI UT WOS:000312824300015 ER PT J AU Campisi, J AF Campisi, J. TI OXIDATIVE DAMAGE: CELLULAR DAMAGE RESPONSES LINK AGING, AGE-RELATED DISEASE, AND INFLAMMATION SO GERONTOLOGIST LA English DT Meeting Abstract C1 [Campisi, J.] Buck Inst Res Aging, Novato, CA USA. [Campisi, J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. NR 0 TC 0 Z9 0 U1 0 U2 2 PU OXFORD UNIV PRESS INC PI CARY PA JOURNALS DEPT, 2001 EVANS RD, CARY, NC 27513 USA SN 0016-9013 J9 GERONTOLOGIST JI Gerontologist PD NOV PY 2012 VL 52 SU 1 BP 405 EP 405 PG 1 WC Gerontology SC Geriatrics & Gerontology GA 061ZG UT WOS:000312888203170 ER PT J AU LaBarge, MA AF LaBarge, M. A. TI AGING MAKES HUMAN MAMMARY GLAND MORE VULNERABLE TO CANCER SO GERONTOLOGIST LA English DT Meeting Abstract C1 [LaBarge, M. A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. NR 0 TC 0 Z9 0 U1 0 U2 2 PU OXFORD UNIV PRESS INC PI CARY PA JOURNALS DEPT, 2001 EVANS RD, CARY, NC 27513 USA SN 0016-9013 J9 GERONTOLOGIST JI Gerontologist PD NOV PY 2012 VL 52 SU 1 BP 608 EP 608 PG 1 WC Gerontology SC Geriatrics & Gerontology GA 061ZG UT WOS:000312888204258 ER PT J AU Nutaro, J Protopopescu, V AF Nutaro, James Protopopescu, Vladimir TI A New Model of Frequency Delay in Power Systems SO IEEE TRANSACTIONS ON CIRCUITS AND SYSTEMS II-EXPRESS BRIEFS LA English DT Article DE Electromechanical waves; frequency sensor; power systems ID PROPAGATION AB Observations of slow frequency signals in power systems have been explained by continuum wave equations that approximate the system's electromechanical dynamics. These continuum models predict that the signal speed is a function of the rotational inertia of the generators and impedances of the transmission lines. Here, we show that frequency signals with speeds modulated by these factors are predicted by the swing and Kirchhoff equations, without resorting to a continuum model. Our analysis also shows that the precision of the sensors used to measure frequency has a significant impact on the apparent speed of the frequency signal. C1 [Nutaro, James; Protopopescu, Vladimir] Oak Ridge Natl Lab, Computat Sci & Engn Div, Oak Ridge, TN 37831 USA. RP Nutaro, J (reprint author), Oak Ridge Natl Lab, Computat Sci & Engn Div, Oak Ridge, TN 37831 USA. EM nutarojj@ornl.gov; protopopesva@ornl.gov OI Nutaro, James/0000-0001-7360-2836 FU Laboratory Directed Research and Development Program of Oak Ridge National Laboratory [DE-AC05-00OR22725]; U.S. Department of Energy [DE-AC05-00OR22725] FX This work was supported by the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory under Contract DE-AC05-00OR22725. This brief was recommended by Associate Editor K.-H. Chen.; This brief has been authored by UT-Battelle, LLC, under Contract DE-AC05-00OR22725, with the U.S. Department of Energy. By accepting the article for publication, the publisher acknowledges that the U.S. Government retains a nonexclusive, paid-up, irrevocable, and worldwide license to publish or reproduce the published form of this brief or allow others to do so, for the U.S. Government purposes. NR 12 TC 3 Z9 4 U1 0 U2 5 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 1549-7747 J9 IEEE T CIRCUITS-II JI IEEE Trans. Circuits Syst. II-Express Briefs PD NOV PY 2012 VL 59 IS 11 BP 840 EP 844 DI 10.1109/TCSII.2012.2220677 PG 5 WC Engineering, Electrical & Electronic SC Engineering GA 069HO UT WOS:000313426100029 ER PT J AU Kshirsagar, P Burgos, RP Jang, J Lidozzi, A Wang, F Boroyevich, D Sul, SK AF Kshirsagar, Parag Burgos, Rolando P. Jang, Jihoon Lidozzi, Alessandro Wang, Fei Boroyevich, Dushan Sul, Seung-Ki TI Implementation and Sensorless Vector-Control Design and Tuning Strategy for SMPM Machines in Fan-Type Applications SO IEEE TRANSACTIONS ON INDUSTRY APPLICATIONS LA English DT Article DE Luenberger observer; sensorless; SMPM; vector control ID MOTOR; DRIVES; SPEED; PMSM; POSITION AB This paper presents a complete design methodology for the sensorless vector control of permanent-magnet synchronous machine (PMSM) motor drives in fan-type applications. The proposed strategy is built over a linear asymptotic state observer used to estimate the PMSM back EMF and a novel tracking controller based on a phase-locked loop system, which, by synchronizing the estimated and actual d-q frames, estimates the rotor speed and position. This paper presents the complete derivation of all associated control loops, namely, state observer; tracking controller; d-q-axis current regulator; speed controller; an antisaturation control loop, which provides inherent operation in the flux-weakening region; and all corresponding antiwindup loops. Detailed design rules are provided for each of these loops, respectively verified through time-domain simulations, frequency-response analysis, and experimental results using a three-phase 7.5-kW PMSM motor drive, validating both the design methodology and the expected performance attained by the proposed control strategy. C1 [Kshirsagar, Parag] United Technol Res Ctr, E Hartford, CT 06108 USA. [Kshirsagar, Parag; Boroyevich, Dushan] Virginia Polytech Inst & State Univ, Blacksburg, VA 24061 USA. [Burgos, Rolando P.] US Corp Res Ctr, ABB Corp Res, Raleigh, NC 27606 USA. [Jang, Jihoon] Gen Motors Adv Technol Ctr, Torrance, CA 90505 USA. [Lidozzi, Alessandro] Roma Tre Univ, I-00154 Rome, Italy. [Wang, Fei] Univ Tennessee, Knoxville, TN 37996 USA. [Wang, Fei] Oak Ridge Natl Lab, Oak Ridge, TN USA. [Sul, Seung-Ki] Seoul Natl Univ, Seoul 151744, South Korea. RP Kshirsagar, P (reprint author), United Technol Res Ctr, E Hartford, CT 06108 USA. EM kshirsp@utrc.utc.com; rburgos@ieee.org; jihoon.s.jang@gmail.com; lidozzi@uniroma3.it; fred.wang@utk.edu; dushan@vt.edu; sulsk@plaza.snu.ac.kr RI Lidozzi, Alessandro/O-7816-2014 OI Lidozzi, Alessandro/0000-0002-8706-8117 FU National Science Foundation (NSF) [EEC-9731677]; Center for Power Electronics Systems Industry Partnership Program FX Manuscript received December 28, 2011; revised April 25, 2012; accepted May 14, 2012. Date of publication November 16, 2012; date of current version December 31, 2012. Paper 2011-IDC-797.R1, presented at the 2006 IEEE Industry Applications Society Annual Meeting, Tampa, FL, October 8-12, and approved for publication in the IEEE TRANSACTIONSON INDUSTRY APPLICATIONS by the Industrial Drives Committee of the IEEE Industry Applications Society. This work was supported in part by the National Science Foundation (NSF) under NSF Award EEC-9731677 and in part by the Center for Power Electronics Systems Industry Partnership Program. NR 14 TC 24 Z9 25 U1 1 U2 18 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0093-9994 J9 IEEE T IND APPL JI IEEE Trans. Ind. Appl. PD NOV-DEC PY 2012 VL 48 IS 6 SI SI BP 2402 EP 2413 DI 10.1109/TIA.2012.2227135 PG 12 WC Engineering, Multidisciplinary; Engineering, Electrical & Electronic SC Engineering GA 068JW UT WOS:000313364000065 ER PT J AU Mandic, G Nasiri, A Muljadi, E Oyague, F AF Mandic, Goran Nasiri, Adel Muljadi, Eduard Oyague, Francisco TI Active Torque Control for Gearbox Load Reduction in a Variable-Speed Wind Turbine SO IEEE TRANSACTIONS ON INDUSTRY APPLICATIONS LA English DT Article DE Gearbox; stress control; variable-speed drives; wind energy; wind turbine ID VIBRATION SUPPRESSION; DRIVE SYSTEM; DISTURBANCE REJECTION; FEEDBACK AB With the advent of power electronics, the size, weight, and cost of power converters have been drastically reduced while efficiency is improved. The use of variable-speed wind power generators has seen considerable growth. The use of gearboxes in the wind turbines allows for smaller size, lower weight, and higher speed generators. However, gearboxes have shown to be one of the least reliable components of the wind turbines. In this paper, we propose a method that can extend the life and reliability of wind turbine gearboxes by reducing the mechanical stress on gearbox components. Reduction of mechanical stress is achieved by the generator torque control that minimizes resonant torsional vibrations within a drivetrain caused by variations in wind velocity. A detailed model for the drivetrain of a 750-kW wind turbine, including a gearbox is presented. Experimental results are used to calculate the parameters of the gearbox. A controller is designed to adjust the generator torque at the end of the drivetrain to remove the unwanted and damaging torque variations from the drivetrain. Simulation results verify the effectiveness of the proposed method. C1 [Mandic, Goran; Nasiri, Adel] Univ Wisconsin, Milwaukee, WI 53201 USA. [Muljadi, Eduard] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Oyague, Francisco] Boulder Wind Power, Boulder, CO 80301 USA. RP Mandic, G (reprint author), Univ Wisconsin, Milwaukee, WI 53201 USA. EM gmandic@uwm.edu; nasiri@uwm.edu; eduard.muljadi@nrel.gov; Francisco.Oyague@boulderwindpower.com FU U.S. Department of Energy [09EE0001386] FX Manuscript received December 16, 2011; revised March 19, 2012; accepted March 28, 2012. Date of publication November 16, 2012; date of current version December 31, 2012. Paper 2011-EMC-779.R1, presented at the 2011 IEEE Energy Conversion Congress and Exposition, Phoenix, AZ, September 17-22, and approved for publication in the IEEE TRANSACTIONS ON INDUSTRY APPLICATIONS by the Electric Machines Committee of the IEEE Industry Applications Society. This work was supported by the U.S. Department of Energy under Award 09EE0001386. NR 27 TC 21 Z9 24 U1 1 U2 19 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0093-9994 J9 IEEE T IND APPL JI IEEE Trans. Ind. Appl. PD NOV-DEC PY 2012 VL 48 IS 6 SI SI BP 2424 EP 2432 DI 10.1109/TIA.2012.2227131 PG 9 WC Engineering, Multidisciplinary; Engineering, Electrical & Electronic SC Engineering GA 068JW UT WOS:000313364000067 ER PT J AU Xiong, LM Deng, Q Tucker, GJ McDowell, DL Chen, YP AF Xiong, Liming Deng, Qian Tucker, Garritt J. McDowell, David L. Chen, Youping TI Coarse-grained atomistic simulations of dislocations in Al, Ni and Cu crystals SO INTERNATIONAL JOURNAL OF PLASTICITY LA English DT Article DE Coarse-grained atomistic simulation; Concurrent atomistic-continuum method; 3D dislocation dynamics; Curved dislocations; Adaptive mesh refinement ID MOLECULAR-DYNAMICS; SINGLE-CRYSTAL; INTERATOMIC POTENTIALS; COUPLED ATOMISTICS; FIELD-THEORY; PLASTICITY; CONTINUUM; DEFORMATION; NUCLEATION; DEFECTS AB This paper presents the application of a recently developed concurrent atomistic continuum (CAC) methodology in coarse-grained (CG) atomistic simulations of dislocation nucleation and migration in face-centered cubic (fcc) Al, Ni and Cu crystals, using an EAM force field and an adaptive mesh refinement strategy. The CAC method is based on recently developed atomistic field theory (AFT) that frames the problem in terms of a continuum field representation of lattice and sublattice atomic arrangements. Four sets of CG models with different finite element mesh refinement are constructed to test the accuracy and efficiency of the CG method relative to full molecular dynamics (MD). Simulation results show that the CG method is able to reproduce key phenomena of dislocation dynamics in initially defect free fcc crystals, including strain bursts caused by dislocation nucleation and migration, the structure of leading and trailing partial dislocations separated by equilibrium stacking faults in Al, formation of intrinsic stacking fault ribbons in Ni and Cu, and 3D migration of curved dislocations, all comparable with results of MD simulations. CG simulations have also revealed that the yield strength of Al depends on the thickness of the specimens as well as the operative deformation mechanisms. The effects of mesh size and adaptive mesh refinement on CG simulation results are analyzed and discussed. (C) 2012 Elsevier Ltd. All rights reserved. C1 [Xiong, Liming; Deng, Qian; Chen, Youping] Univ Florida, Dept Mech & Aerosp Engn, Gainesville, FL 32611 USA. [Tucker, Garritt J.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [McDowell, David L.] Georgia Inst Technol, Sch Mat Sci & Engn, Atlanta, GA 30332 USA. [McDowell, David L.] Georgia Inst Technol, Woodruff Sch Mech Engn, Atlanta, GA 30332 USA. RP Chen, YP (reprint author), Univ Florida, Dept Mech & Aerosp Engn, Gainesville, FL 32611 USA. EM ypchen2@ufl.edu RI Deng, Qian/J-3992-2014; Chen, Youping /G-2931-2010; Tucker, Garritt/A-1954-2016; Xiong, Liming/B-9810-2017 OI Deng, Qian/0000-0003-3556-8897; Chen, Youping /0000-0002-9626-9009; Tucker, Garritt/0000-0002-4011-450X; FU National Science Foundation [CMMI-0758265, CMMI-0855795, CMMI-1129976]; DARPA [N66001-10-1-4018]; Department of Energy [DOE/DE-SC0006539]; US Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This material is based upon the work supported by National Science Foundation under Award Numbers CMMI-0758265 (McDowell), CMMI-0855795 and CMMI-1129976, DARPA under Award Number N66001-10-1-4018, and Department of Energy under Award Number DOE/DE-SC0006539 (Xiong, Deng, and Chen). Any opinions, findings and conclusions or recommendations expressed in this publication are those of the author(s) and do not necessarily reflect the views of the National Science Foundation, DOE or DARPA. Simulations were performed at the High Performance Computing Center at the University of Florida. This research was supported in part by the National Science Foundation through Teragrid resources provided by TACC. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the US Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL85000. NR 53 TC 17 Z9 17 U1 5 U2 43 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0749-6419 J9 INT J PLASTICITY JI Int. J. Plast. PD NOV PY 2012 VL 38 BP 86 EP 101 DI 10.1016/j.ijplas.2012.05.002 PG 16 WC Engineering, Mechanical; Materials Science, Multidisciplinary; Mechanics SC Engineering; Materials Science; Mechanics GA 068QP UT WOS:000313381600005 ER PT J AU Aad, G Abajyan, T Abbott, B Abdallah, J Khalek, SA Abdelalim, AA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Acerbia, E Acharya, BS Adamczyk, L Adams, DL Addy, TN Adelman, J Adomeit, S Adragna, P Adye, T Aefsky, S Aguilar-Saavedra, JA Agustoni, M Aharrouche, M Ahlen, SP Ahles, F Ahmad, A Ahsan, M Aielli, G Akdogan, T Akesson, TPA Akimoto, G Akimov, AV Alam, MS Alam, MA Albert, J Albrand, S Aleksa, M Aleksandrov, IN Alessandria, F Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Aliev, M Alimonti, G Alison, J Allbrooke, BMM Allport, PP Allwood-Spiers, SE Almond, J Aloisio, A Alon, R Alonso, A Alonso, F Gonzalez, BA Alviggi, MG Amako, K Amelung, C Ammosov, VV Amorim, A Amram, N Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Anduaga, XS Anger, P Angerami, A Anghinolfi, F Anisenkov, A Anjos, N Annovi, A Antonaki, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Aoun, S Bella, LA Apolle, R Arabidze, G Aracena, I Arai, Y Arce, ATH Arfaoui, S Arguin, JF Arik, E Arik, M Armbruster, AJ Arnaez, O Arnal, V Arnault, C Artamonov, A Artoni, G Arutinov, D Asai, S Asfandiyarov, R Ask, S Asman, B Asquith, L Assamagan, K Astbury, A Atkinson, M Aubert, B Auge, E Augsten, K Aurousseau, M Avolio, G Avramidou, R Axen, D Azuelos, G Azuma, Y Baak, MA Baccaglioni, G Bacci, C Bach, AM Bachacou, H Bachas, K Backes, M Backhaus, M Badescu, E Bagnaia, P Bahinipati, S Bai, Y Bailey, DC Bain, T Baines, JT Baker, OK Baker, MD Baker, S Banas, E Banerjee, P Banerjee, S Banfi, D Bangert, A Bansal, V Bansil, HS Barak, L Baranov, SP Galtieri, AB Barber, T Barberio, EL Barberis, D Barbero, M Bardin, DY Barillari, T Barisonzi, M Barklow, T Barlow, N Barnett, BM Barnett, RM 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Bingul, A Bini, C Biscarat, C Bittner, B Black, KM Blair, RE Blanchard, JB Blanchot, G Blazek, T Blocker, C Blocki, J Blondel, A Blum, W Blumenschein, U Bobbink, GJ Bobrovnikov, VB Bocchetta, SS Bocci, A Boddy, CR Boehler, M Boek, J Boelaert, N Bogaerts, JA Bogdanchikov, A Bogouch, A Bohm, C Bohm, J Boisvert, V Bold, T Boldea, V Bolnet, NM Bomben, M Bona, M Boonekamp, M Booth, CN Bordoni, S Borer, C Borisov, A Borissov, G Borjanovic, I Borri, M Borroni, S Bortolotto, V Bos, K Boscherini, D Bosman, M Boterenbrood, H Bouchami, J Boudreau, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boveia, A Boyd, J Boyko, IR Bozovic-Jelisavcic, I Bracinik, J Branchini, P Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Brazzale, SF Brelier, B Bremer, J Brendlinger, K Brenner, R Bressler, S Britton, D Brochu, FM Brock, I Brock, R Broggi, F Bromberg, C Bronner, J Brooijmans, G Brooks, T Brooks, WK Brown, G Brown, H De Renstrom, PAB Bruncko, D Bruneliere, R Brunet, S 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De Salvo, A De Sanctis, U De Santo, A De Regie, JBD De Zorzi, G Dearnaley, WJ Debbe, R Debenedetti, C Dechenaux, B Dedovich, DV Degenhardt, J Del Papa, C Del Peso, J Del Prete, T Delemontex, T Deliyergiyev, M Dell'Acqua, A Dell'Asta, L Della Pietra, M della Volpe, D Delmastro, M Delsart, PA Deluca, C Demers, S Demichev, M Demirkoz, B Deng, J Denisov, SP Derendarz, D Derkaoui, JE Derue, F Dervan, P Desch, K Devetak, E Deviveiros, PO Dewhurst, A DeWilde, B Dhaliwal, S Dhullipudi, R Di Ciaccio, A Di Ciaccio, L Di Girolamo, A Di Girolamo, B Di Luise, S Di Mattia, A Di Micco, B Di Nardo, R Di Simone, A Di Sipio, R Diaz, MA Diehl, EB Dietrich, J Dietzsch, TA Diglio, S Yagci, KD Dingfelder, J Dinut, F Dionisi, C Dita, P Dita, S Dittus, F Djama, F Djobava, T do Vale, MAB Wemans, AD Doan, TKO Dobbs, M Dobinson, R Dobos, D Dobson, E Dodd, J Doglioni, C Doherty, T Doi, Y Dolejsi, J Dolenc, I Dolezal, Z Dolgoshein, BA Dohmae, T Donadelli, M Donini, J Dopke, J Doria, A Dos Anjos, A Dotti, A Dova, 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Zhou, B. Zhou, N. Zhou, Y. Zhu, C. G. Zhu, H. Zhu, J. Zhu, Y. Zhuang, X. Zhuravlov, V. Zieminska, D. Zimin, N. I. Zimmermann, R. Zimmermann, S. Zimmermann, S. Ziolkowski, M. Zitoun, R. Zivkovic, L. Zmouchko, V. V. Zobernig, G. Zoccolia, A. Zur Nedden, M. Zutshi, V. Zwalinski, L. CA Atlas Collaboration TI Search for a heavy top-quark partner in final states with two leptons with the ATLAS detector at the LHC SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering ID DYNAMICAL SYMMETRY-BREAKING; ROOT-S=7 TEV; HADRON COLLIDERS; PP COLLISIONS; SUPERGAUGE TRANSFORMATIONS; MEASURING MASSES; SUPERSYMMETRY; MODEL; PERFORMANCE; PARTICLE AB The results of a search for direct pair production of heavy top-quark partners in 4.7 fb(-1) of integrated luminosity from p p collisions at root s = 7 TeV collected by the ATLAS detector at the LHC are reported. Heavy top-quark partners decaying into a top quark and a neutral non-interacting particle are searched for in events with two leptons in the final state. No excess above the Standard Model expectation is observed. Limits are placed on the mass of a supersymmetric scalar top and of a spin-1/2 top-quark partner. A spin-1/2 top-quark partner with a mass between 300 GeV and 480 GeV, decaying to a top quark and a neutral non-interacting particle lighter than 100 GeV, is excluded at 95% confidence level. C1 [Jackson, P.; Onyisi, P. U. E.; Soni, N.] Univ Adelaide, Sch Chem & Phys, Adelaide, SA 5000, Australia. [Alam, M. S.; Edson, W.; Ernst, J.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Bahinipati, S.; Chan, K.; Gingrich, D. M.; Moore, R. W.; Pinfold, J. L.; Subramania, Hs.; Vives Vaque, F.] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakir, O.; Ciftci, A. K.; Ciftci, R.; Yildiz, H. Duran; Kuday, S.] Ankara Univ, Dept Phys, TR-06100 Ankara, Turkey. 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S.; Bracinik, J.; Charlton, D. G.; Chisholm, A. S.; Collins, N. J.; Curtis, C. J.; Hadley, D. R.; Hawkes, C. M.; Head, S. J.; Hillier, S. J.; Mahout, G.; Martin, T. A.; Mclaughlan, T.; Newman, P. R.; Nikolopoulos, K.; O'Neale, S. W.; Palmer, J. D.; Slater, M.; Thomas, J. P.; Thompson, P. D.; Watkins, P. M.; Watson, A. T.; Watson, M. F.; Wilson, J. A.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Akdogan, T.; Arik, E.; Arik, M.; Istin, S.; Ozcan, V. E.; Rador, T.; Vercesia, V.] Bogazici Univ, Dept Phys, Istanbul, Turkey. [Cetin, S. A.] Dogus Univ, Div Phys, Istanbul, Turkey. [Beddall, A. J.; Beddall, A.; Bingul, A.] Gaziantep Univ, Dept Engn Phys, Gaziantep, Turkey. Istanbul Tech Univ, Dept Phys, TR-80626 Istanbul, Turkey. [Bellagamba, L.; Bertin, A.; Bindi, M.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; Caforio, D.; Ciocca, C.; Corradi, M.; De Castro, S.; Di Sipio, R.; Fabbri, L.; Franchini, M.; Giacobbe, B.; Giusti, P.; Grafstrom, P.; Jha, M. K.; Massaa, I.; Mengarelli, A.; Monzani, S.; Negrini, M.; Piccinini, M.; Polini, A.; Rinaldi, L.; Romano, M.; Sbarra, C.; Sbrizzi, A.; Semprini-Cesari, N.; Spighia, R.; Valentinetti, S.; Villa, M.; Zoccolia, A.] Univ Bologna, Ist Nazl Fis Nucl, Sez Bologna, Bologna, Italy. [Bertin, A.; Bindi, M.; Caforio, D.; Ciocca, C.; De Castro, S.; Di Sipio, R.; Fabbri, L.; Massaa, I.; Mengarelli, A.; Monzani, S.; Piccinini, M.; Romano, M.; Sbrizzi, A.; Semprini-Cesari, N.; Valentinetti, S.; Villa, M.; Zoccolia, A.] Univ Bologna, Dipartimento Fis, Bologna, Italy. [Abajyan, T.; Arutinov, D.; Backhaus, M.; Barbero, M.; Bechtle, P.; Brock, I.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Gaycken, G.; Geich-Gimbel, Ch.; Gonella, L.; Haefner, P.; Havranek, M.; Hellmich, D.; Hillert, S.; Huegging, F.; Ince, T.; Karagounis, M.; Khoriauli, G.; Koevesarki, P.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lapoire, C.; Lehmacher, M.; Leyko, A. M.; Limbach, C.; Loddenkoetter, T.; Mazur, M.; Moeser, N.; Mueller, K.; Nanava, G.; Nattermann, T.; Nuncio-Quiroz, A. -E.; Pohl, D.; Psoroulas, S.; Schaepe, S.; Schmieden, K.; Schmitz, M.; Schultens, M. J.; Schwindt, T.; Stillings, J. A.; Therhaag, J.; Tsung, J. -W.; Uchida, K.; Uhlenbrock, M.; Vogel, A.; Von Toerne, E.; Wang, T.; Wermes, N.; Wienemann, P.; Zendler, C.; Zimmermann, R.; Zimmermann, S.] Univ Bonn, Inst Phys, Bonn, Germany. [Ahlen, S. P.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, Boston, MA 02215 USA. [Aefsky, S.; Amelung, C.; Bensinger, J. R.; Blocker, C.; Daya-Ishmukhametova, R. K.; Gozpinar, S.; Pomeroy, D.; Sciolla, G.; Wellenstein, H.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Perantoni, M.; Seixas, J. M.] Univ Fed Rio de Janeiro, COPPE, EE, IF, Rio De Janeiro, Brazil. [Cerqueira, A. 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[Alexa, C.; Badescu, E.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Cuciuc, C. -M.; Dinut, F.; Dita, P.; Dita, S.; Micu, L.; Olariu, A.; Pantea, D.; Popeneciu, G. A.; Rotaru, M.; Spousta, M.; Stoicea, G.; Tudorachea, A.; Tudorachea, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Darlea, G. L.] Univ Politehn Bucuresti, Bucharest, Romania. W Univ Timisoara, Timisoara, Romania. [Silva, M. L. Gonzalez; Otero y Garzon, G.; Piegaia, R.; Romeo, G.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Ask, S.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Buttinger, W.; Carter, J. R.; Chapman, J. D.; Cowden, C.; French, S. T.; Frost, J. A.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Moeller, V.; Parker, M. A.; Robinson, D.; Sandoval, T.; Thomson, M.; Ward, C. P.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Gillberg, D.; Koffas, T.; Liu, C.; Marchand, J. F.; McCarthy, T. G.; Oakham, F. G.; Randrianarivony, K.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Anastopoulos, C.; Anghinolfi, F.; Baak, M. A.; Bachas, K.; Banfi, D.; Battistin, M.; Bellina, F.; Bellomo, M.; Beltramello, O.; Berge, D.; Bianchi, R. M.; Blanchot, G.; Bogaerts, J. A.; Boyd, J.; Bremer, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Catmore, J. R.; Cattai, A.; Cerri, A.; Barajas, C. A. Chavez; Childers, J. T.; Chromek-Burckhart, D.; Cote, D.; Danielsson, H. O.; Dell'Acqua, A.; Di Girolamo, A.; Di Girolamo, B.; Di Micco, B.; Dittus, F.; Dobinson, R.; Dobos, D.; Dobson, E.; Dopke, J.; Dudarev, A.; Uhrssen, M. D.; Dunford, M.; Dydak, F.; Ellis, N.; Elsing, M.; Fabre, C.; Farthouat, P.; Fassnacht, P.; Francis, D.; Franz, S.; Froeschl, R.; Froidevaux, D.; Torregrosa, E. Fullana; Gabaldon, C.; Garelli, N.; Garonne, V.; Gianotti, F.; Gibson, S. 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O.; Schlenker, S.; Schott, M.; Sfyrla, A.; Spigo, G.; Spiwoks, R.; Stewart, G. A.; Teischinger, F. A.; Ten Kate, H.; Torchiani, I.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van der Ster, D.; Van Eldik, N.; Vandelli, W.; Veness, R.; Vinek, E.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Winklmeier, F.; Wotschack, J.; Byszewski, M.; Zajacova, Z.; Zwalinski, L.] CERN, Geneva, Switzerland. [Anderson, K. J.; Boveia, A.; Canellig, F.; Choudalakis, G.; Fiascaris, M.; Gardner, R. W.; Jen-La Plante, I.; Kapliy, A.; Melachrinos, C.; Merritt, F. S.; Meyer, C.; Miller, D. W.; Okumura, Y.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Shochet, M. J.; Tompkins, L.; Tuggle, J. M.; Vukotic, I.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Diaz, M. A.; Pino, S. A. Olivares; Quinonez, F.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Carquin, E.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Jin, S.; Lu, F.; Ouyang, Q.; Ruan, X.; Shan, L. Y.; Yao, L.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Han, L.; Jiang, Y.; Li, S.; Liu, M.; Liu, Y.; Peng, H.; Wang, H.; Wu, Y.; Xu, C.; Zhang, D.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Toro, R. Camacho; Cinca, D.; Donini, J.; Febbraro, R.; Ghodbane, N.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Vazeille, F.] Clermont Univ, Phys Corpusculaire Lab, Aubiere, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Toro, R. Camacho; Cinca, D.; Donini, J.; Febbraro, R.; Liao, H.; Pallin, D.; Hernandez, D. 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Bruckman; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Malecki, P.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Turala, M.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.; Zemla, A.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Yagci, K. Dindar; Firan, A.; Hadavand, H. K.; Hoffman, J.; Ishmukhametov, R.; Joffe, D.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Rios, R. R.; Sekula, S. J.; Stroynowski, R.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Ahsan, M.; Izen, J. M.; Lou, X.; Reeves, K.; Wong, W. C.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Kuutmann, E. Bergeaas; Dassoulas, J. A.; Dietrich, J.; Ehrenfeld, W.; Ferrara, V.; Fischer, G.; Friedrich, C.; Glazov, A.; Goebel, M.; Fajardo, L. S. Gomez; Goncalves Pinto Firmino Da Costa, J.; Gosdzik, B.; Grahn, K-J.; Gregor, I. M.; Hiller, K. 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A.; Zhu, H.] DESY, Zeuthen, Germany. [Bunse, M.; Esch, H.; Goessling, C.; Gossling, C.; Hirsch, F.; Jung, C. A.; Klingenberg, R.; Reisinger, I.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Abdinov, O.; Anger, P.; Czodrowski, P.; Friedrich, F.; Goepfert, T.; Kobel, M.; Leonhardt, K.; Ludwig, A.; Mader, W. F.; Morgenstern, M.; Prudent, X.; Rudolph, C.; Schnoor, U.; Schwierz, R.; Seifert, F.; Steinbach, P.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Ko, B. R.; Kotwal, A.; Oh, S. H.; Wang, C.; Yamaoka, J.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Buckley, A. G.; Clark, P. J.; Debenedetti, C.; Harrington, R. D.; Martin, V. J.; O'Brien, B. J.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Cerutti, F.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.; Volpi, G.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Aad, G.; Ahles, F.; Barber, T.; Bernhard, R.; Boehler, M.; Bruneliere, R.; Christov, A.; Consorti, V.; Fehling-Kaschek, M.; Flechl, M.; Glatzer, J.; Glatzer, J.; Hartert, J.; Herten, G.; Horner, S.; Jakobs, K.; Janus, M.; Kollefrath, M.; Kononov, A. I.; Kuehn, S.; Lai, S.; Landgraf, U.; Lohwasser, K.; Ludwig, I.; Ludwig, J.; Lumb, D.; Mahboubi, K.; Mohr, W.; Nilsen, H.; Parzefall, U.; Rammensee, M.; Rave, T. C.; Rurikova, Z.; Schmidt, E.; Schumacher, M.; Siegert, F.; Stoerig, K.; Sundermann, J. E.; Temming, K. K.; Thoma, S.; Tsiskaridze, V.; Venturi, M.; Vivarelli, I.; Von Radziewski, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Wiik-Fuchs, L. A. M.; Winkelmann, S.; Xie, S.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, D-79106 Freiburg, Germany. [Abdelalim, A. A.; Alexandre, G.; Backes, M.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; Blondel, A.; Bucci, F.; Clark, A.; Dao, V.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Iacobucci, G.; La Rosa, A.; Lister, A.; Latour, B. Martin Dit; Mermod, P.; Herrera, C. Mora; Nektarijevic, S.; Nikolics, K.; Pasztor, G.; Picazio, A.; Pohl, M.; Rosbach, K.; Rosselet, L.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Beccherle, R.; Caso, C.; Dameri, M.; Darbo, G.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Barberis, D.; Caso, C.; Dameri, M.; Parodi, A. Ferretto; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Chikovani, L.; Tskhadadze, E. G.] Tbilisi State Univ, E Andronikashvili Inst Phys, GE-380086 Tbilisi, Rep of Georgia. [Djobava, T.; Khubua, J.; Mchedlidze, G.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Duren, M.; Stenzel, H.] Univ Giessen, Inst Phys 2, D-6300 Giessen, Germany. [Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Bussey, P.; Buttar, C. M.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Edwards, N. C.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Kar, D.; Kenyon, M.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Robson, A.; Saxon, D. H.; Smith, K. M.; St. Denis, R. D.; Steele, G.; Thompson, A. S.; Wraight, K.; Wright, M.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bierwagen, K.; Blumenschein, U.; Brandt, O.; Erdmann, J.; Evangelakou, D.; George, M.; Grosse-Knetter, J.; Guindon, S.; Haller, J.; Hamer, M.; Henrichs, A.; Hensel, C.; Keil, M.; Knue, A.; Kohn, F.; Krieger, N.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Mann, A.; Meyer, J.; Morel, J.; Pashapour, S.; Quadt, A.; Roe, A.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Uhrmacher, M.; Vazquez Schroeder, T.; Weber, P.; Weingarten, J.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Stark, J.; Sun, X.; Trocme, B.; Wang, J.; Weydert, C.] Univ Grenoble 1, Lab Phys Subatom & Cosmol, Grenoble, France. [Albrand, S.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Stark, J.; Sun, X.; Trocme, B.; Wang, J.; Weydert, C.] CNRS, IN2P3, Grenoble, France. [Albrand, S.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Stark, J.; Sun, X.; Trocme, B.; Wang, J.; Weydert, C.] Inst Natl Polytech Grenoble, F-38031 Grenoble, France. [Addy, T. N.; Harvey, A.; McFarlane, K. W.; Shin, T.; Vassilakopoulos, V. I.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Da Costa, J. Barreiro Guimaraes; Belloni, A.; Catastini, P.; Conti, G.; Huth, J.; Jeanty, L.; Kagan, M.; Mateos, D. Lopez; Outschoorn, V. Martinez; Mercurio, K. M.; Mills, C.; Morii, M.; Skottowe, H. P.; Smith, B. C.; Zevi Della Porta, G.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Anders, G.; Andrei, V.; Davygora, Y.; Dietzsch, T. A.; Geweniger, C.; Hanke, P.; Henke, M.; Khomich, A.; Kluge, E. -E.; Langa, V. S.; Lendermann, V.; Lepold, F.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Stamena, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, D-6900 Heidelberg, Germany. [Kugel, A.; Maenner, R.; Schroer, N.] Heidelberg Univ, ZITI Inst Tech Informat, D-6800 Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Cwetanski, P.; Evans, H.; Gagnon, P.; Jain, V.; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Price, D.; Whittington, D.; Yang, Y.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Epp, B.; Jussel, P.; Kneringer, E.; Kuhn, D.; Lukas, W.; Rudolph, G.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Limper, M.; Mallik, U.; Pylypchenko, Y.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Rosenberg, E. I.; Ruiz-Martinez, A.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Aleksandrov, I. N.; Bardin, D. Y.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Grigalashvili, N.; Huseynov, N.; Kalinovskaya, L. V.; Kazarinov, M. Y.; Kekelidze, G. D.; Kharchenko, D.; Khramov, E.; Kolesnikov, V.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Pozdnyakov, V.; Rumyantsev, L.; Rusakovich, N. A.; Sadykov, R.; Shiyakova, M.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.; Zimin, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Arai, Y.; Doi, Y.; Haruyama, T.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Makida, Y.; Manabe, A.; Mitsui, S.; Nagano, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Hayakawa, T.; King, M.; Kishimoto, T.; Kitamura, T.; Kurashige, H.; Matsushita, T.; Ochi, A.; Suzuki, Y.; Takeda, H.; Tani, K.; Watanabe, I.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Sasao, N.; Sumida, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kantserov, V. A.; Kawagoe, K.; Oda, S.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Univ Nacl La Plata, Inst Fis Plata, La Plata, Buenos Aires, Argentina. [Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Davidson, R.; de Mora, L.; Dearnaley, W. J.; Fox, H.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Bianco, M.; Cataldi, G.; Chiodini, G.; Gorini, E.; Grancagnolo, F.; Orlando, N.; Perrino, R.; Primavera, M.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Bianco, M.; Orlando, N.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Greenshaw, T.; Gwilliam, C. B.; Hayward, H. S.; Jackson, J. N.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kluge, T.; Kretzschmar, J.; Laycock, P.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Sellers, G.; Vossebeld, J. H.; Waller, P.; Wrona, B.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Dolenc, I.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Dolenc, I.; Filipcic, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia. [Adragna, P.; Bona, M.; Carter, A. A.; Cerrito, L.; Eisenhandler, E.; Ellis, K.; Goddard, J. R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Poll, J.; Rizvi, E.; Salamanna, G.; Castanheira, M. Teixeira Dias; Wiglesworth, C.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Alam, M. A.; Berry, T.; Boisvert, V.; Brooks, T.; Cantrill, R.; Cowan, G.; Duguid, L.; Edwards, C. A.; George, S.; Goncalo, R.; Goncalo, R.; Hayden, D.; Pastore, Fr.; Rose, M.; Spano, F.; Strong, J. A.; Teixeira-Dias, P.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Baker, S.; Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Chislett, R. T.; Christidi, I. A.; Cooper, B. D.; Davison, A. R.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Lambourne, L.; Monk, J.; Nash, M.; Nurse, E.; Prabhu, R.; Sherwood, P.; Simmons, B.; Taylor, C.; Waugh, B. M.; Wijeratne, A.] UCL, Dept Phys & Astron, London, England. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Cavalleri, P.; Chareyre, E.; Davignon, O.; De Cecco, S.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph.; Theveneaux-Pelzer, T.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Cavalleri, P.; Chareyre, E.; Davignon, O.; De Cecco, S.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph.; Theveneaux-Pelzer, T.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Cavalleri, P.; Chareyre, E.; Davignon, O.; De Cecco, S.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph.; Theveneaux-Pelzer, T.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Alonso, A.; Bocchetta, S. S.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Jarlskog, G.; Lundberg, B.; Lytken, E.; Meirose, B.; Mjornmark, J. U.; Smirnova, O.] Lund Univ, Inst Fys, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Labarga, L.; Lagouri, T.; Merino, J. Llorente; March, L.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Aharrouche, M.; Arnaez, O.; Blum, W.; Brau, B.; Buscher, V.; Caputo, R.; Eckweiler, S.; Ellinghaus, F.; Ertel, E.; Fiedler, F.; Fleckner, J.; Goeringer, C.; Handel, C.; Hohlfeld, M.; Hsu, P. J.; Ji, W.; Kawamura, G.; Kleinknecht, K.; Koenig, S.; Kopke, L.; Lungwitz, M.; Mattig, S.; Masetti, L.; Meyer, C.; Moreno, D.; Mueller, T.; Neusiedl, A.; Sander, H. G.; Schafer, U.; Schmitt, C.; Schroeder, C.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.] Johannes Gutenberg Univ Mainz, Inst Phys, D-6500 Mainz, Germany. [Almond, J.; Borri, M.; Brown, G.; Chavda, V.; Cox, B. E.; Da Via, C.; Duerdoth, I. P.; Forti, A.; Howarth, J.; Ibbotson, M.; Joshi, K. D.; Klinger, J. A.; Lane, J. L.; Loebinger, F. K.; Marx, M.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Pilkington, A. D.; Robinson, J. E. M.; Schwanenberger, C.; Snow, S. W.; Watts, S.; Woudstra, M. J.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aoun, S.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Odier, J.; Pralavorio, P.; Rozanov, A.; Talby, M.; Tannoury, N.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aoun, S.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Maurer, J.; Monnier, E.; Odier, J.; Pralavorio, P.; Rozanov, A.; Talby, M.; Tannoury, N.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Brau, B.; Colon, G.; Dallapiccola, C.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Caron, B.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Dobbs, M.; Dufour, M-A.; Guler, H.; Klemetti, M.; Mc Donald, J.; Robertsonk, S. H.; Santamarina Rios, C.; Schram, M.; Stockton, M. C.; Vachon, B.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Davidson, N.; Diglio, S.; Jennens, D.; Kubota, T.; Limosani, A.; Moorhead, G. F.; Hanninger, G. Nunes; Phan, A.; Shao, Q. T.; Taylor, G. N.; Thong, W. M.; Volpi, M.; White, M. J.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Armbruster, A. J.; Borroni, S.; Chapman, J. W.; Cirilli, M.; Dai, T.; Diehl, E. B.; Ferretti, C.; Goldfarb, S.; Harper, D.; Levin, D.; Li, X.; Liu, H.; Liu, J. B.; Liu, L.; Mc Kee, S. P.; Neal, H. A.; Panikashvili, N.; Purdham, J.; Qian, J.; Scheirich, D.; Thun, R. P.; Walch, S.; Wilson, A.; Wooden, G.; Yang, H.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Fedorko, W.; Hauser, R.; Heim, S.; Holzbauer, J. L.; Huston, J.; Koll, J.; Linnemann, J. T.; Mangeard, P. S.; Martin, B.; Miller, R. J.; Pope, B. G.; Schwienhorst, R.; Stelzer, H. J.; Tollefson, K.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Acerbia, E.; Alessandria, F.; Alimonti, G.; Andreazza, A.; Baccaglioni, G.; Besana, M. I.; Broggi, F.; Carminati, L.; Cavalli, D.; Citterio, M.; Consonni, S. M.; Costa, G.; Fanti, M.; Favareto, A.; Giugni, D.; Koletsou, I.; Lari, T.; Mandelli, L.; Mazzanti, M.; Meloni, F.; Meronia, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Rivoltella, G.; Simoniello, R.; Tartarellia, G. F.; Troncona, C.; Turra, R.; Vegni, G.; Volpinia, G.] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Acerbia, E.; Andreazza, A.; Besana, M. I.; Carminati, L.; Consonni, S. M.; Fanti, M.; Favareto, A.; Meloni, F.; Perini, L.; Pizio, C.; Ragusa, F.; Rivoltella, G.; Simoniello, R.; Turra, R.; Vegni, G.] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Harkusha, S.; Kurochkin, Y. A.; Satsounkevitch, I.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus. [Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Azuelos, G.; Banerjee, P.; Bouchami, J.; Davies, M.; Giunta, M.; Leroy, C.; Martin, J. P.; Mehdiyev, R.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.] Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Khodinov, A.; Leroy, C.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.] Moscow Engn & Phys Inst MEPhI, Moscow, Russia. [Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Beale, S.; Becker, S.; Biebel, O.; Calfayan, P.; de Graat, J.; Duckeck, G.; Ebke, J.; Elmsheuser, J.; Engl, A.; Galea, C.; Heller, C.; Hertenberger, R.; Kummer, C.; Legger, F.; Lichtnecker, M.; Lorenz, J.; Mameghani, R.; Mueller, T. A.; Nunnemann, T.; Oakes, L. B.; Rauscher, F.; Reznicek, P.; Sanders, M. P.; Schaile, D.; Schieck, J.; Serfon, C.; Staude, A.; Vladoiu, D.; Walker, R.; Will, J. Z.; Zhuang, X.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Beimforde, M.; Bethke, S.; Bittner, B.; Bronner, J.; Capriotti, D.; Cortiana, G.; Dubbert, J.; Flowerdew, M. J.; Giovannini, P.; Jantsch, A.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kotov, S.; Kroha, H.; Macchiolo, A.; Manfredini, A.; Menke, S.; Moser, H. G.; Nagel, M.; Nisius, R.; Oberlack, H.; Pahl, C.; Pospelov, G. E.; Potrap, I. N.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Seuster, R.; Stern, S.; Stonjek, S.; Vanadia, M.; Von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.; Zhuravlov, V.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Shimizu, S.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Shimizu, S.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Capasso, L.; Carlino, G.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; della Volpe, D.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Musto, E.; Patricelli, S.; Sanchez, A.; Sekhniaidze, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Capasso, L.; Chiefari, G.; della Volpe, D.; Merola, L.; Musto, E.; Patricelli, S.; Sanchez, A.] Univ Naples Federico II, Dipartimento Sci Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Chelstowska, M. A.; De Groot, N.; Filthaut, F.; Klok, P. F.; Koenig, A. C.; Koetsveld, F.; Raas, M.; Salvucci, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Doxiadis, A. D.; Ferrari, P.; Garitaonandia, H.; Geerts, D. A. A.; Gosselink, M.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kayl, M. S.; Klous, S.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Luijckx, G.; Massaro, G.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Pani, P.; Rijpstra, M.; Ruckstuhl, N.; Ta, D.; Tsiakiris, M.; Turlay, E.; Van der Deijl, P. C.; Van der Geer, R.; van der Graaf, H.; van der Leeuw, R.; van der Poel, E.; Van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Doxiadis, A. D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kayl, M. S.; Klous, S.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Luijckx, G.; Massaro, G.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Pani, P.; Rijpstra, M.; Ruckstuhl, N.; Ta, D.; Tsiakiris, M.; Turlay, E.; Van der Deijl, P. C.; Van der Geer, R.; van der Graaf, H.; van der Leeuw, R.; van der Poel, E.; Van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.] Univ Amsterdam, Amsterdam, Netherlands. [Calkins, R.; Chakraborty, D.; Cole, S.; de Lima, J. G. Rocha; Suhr, C.; Yurkewicz, A.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A.; Beloborodova, O.; Bobrovnikov, V. B.; Bogdanchikov, A.; Kazanin, V. A.; Kolachev, G. M.; Korol, A.; Malyshev, V.; Maslennikov, A. L.; Orlov, I.; Peleganchuk, S. V.; Schamov, A. G.; Skovpen, K.; Soukharev, A.; Talyshev, A.; Tikhonov, Y. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Budick, B.; Casadei, D.; Cranmer, K.; van Huysduynen, L. Hooft; Kaplan, B.; Konoplich, R.; Krasznahorkay, A.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.; Prokofiev, K.; Shibata, A.; Zhao, L.] NYU, Dept Phys, New York, NY 10003 USA. [Fisher, M. J.; Gan, K. K.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Rahimi, A. M.; Strang, M.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Gutierrez, P.; Jana, D. K.; Marzin, A.; Meera-Lebbai, R.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Snow, J.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Khanov, A.; Rizatdinova, F.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Hamal, P.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Potter, C. T.; Ptacek, E.; Radloff, P.; Reinsch, A.; Searcy, J.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Andari, N.; Arnault, C.; Auge, E.; Barrillon, P.; Benoit, M.; Binet, S.; Bourdarios, C.; De la Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Grivaz, J. -F.; Fournier, D.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Matricon, P.; Niedercorn, F.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Teinturier, M.; Veillet, J. J.; Wicek, F.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Andari, N.; Arnault, C.; Auge, E.; Barrillon, P.; Benoit, M.; Binet, S.; Bourdarios, C.; De la Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Matricon, P.; Niedercorn, F.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Teinturier, M.; Veillet, J. J.; Wicek, F.; Zerwas, D.; Zhang, Z.] CNRS, IN2P3, F-91405 Orsay, France. [Hanagaki, K.; Hirose, M.; Lee, J. S. H.; Meguro, T.; Nomachi, M.; Sugaya, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Buran, T.; Cameron, D.; Gjelsten, B. K.; Lund, E.; Ould-Saada, F.; Pajchel, K.; Read, A. L.; Rohne, O.; Samset, B. H.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Apolle, R.; Barr, A. J.; Boddy, C. R.; Brandt, G.; Buchanan, J.; Buckingham, R. M.; Coniavitis, E.; Cooper-Sarkar, A. M.; Dafinca, A.; Davies, E.; Gwenlan, C.; Hall, D.; Hays, C. P.; Howard, J.; Huffman, T. B.; Issever, C.; King, R. S. B.; Kogan, L. A.; Korn, A.; Larner, A.; Lewis, A.; Liang, Z.; Livermore, S. S. A.; Mattravers, C.; Nickerson, R. B.; Pinder, A.; Robichaud-Veronneau, A.; Ryder, N. C.; Short, D.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Whitehead, S. R.; Young, C. J.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Colombo, T.; Conta, C.; Ferrari, R.; Franchino, S.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Uslenghi, M.; Vercesia, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Colombo, T.; Conta, C.; Franchino, S.; Livan, M.; Negri, A.; Rebuzzi, D. M.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Alison, J.; Brendlinger, K.; Degenhardt, J.; Fratina, S.; Hines, E.; Hong, T. M.; Jackson, B.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Olivito, D.; Ospanov, R.; Reece, R.; Saxon, J.; Schaefer, D.; Stahlman, J.; Thomson, E.; Wagner, P.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Bertolucci, F.; Cascella, M.; Cavasinni, V.; Crescioli, F.; Del Prete, T.; Dotti, A.; Roda, C.; Sarri, F.; White, S.; Zinonos, Z.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Bertolucci, F.; Cascella, M.; Cavasinni, V.; Crescioli, F.; Del Prete, T.; Dotti, A.; Roda, C.; Sarri, F.; White, S.; Zinonos, Z.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Boudreau, J.; Cleland, W.; Escobar, C.; Kittelmann, T.; Mueller, J.; Prieur, D.; Rescigno, M.; Savinov, V.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amorim, A.; Anjos, N.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Wemans, A. Do Valle; Fiolhais, M. C. N.; Gomes, A.; Jorge, P. M.; Lopes, L.; Miguens, J. Machado; Maio, A.; Maneira, J.; Oliveira, M.; Onofre, A.; Palma, A.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Aguilar-Saavedra, J. A.; Amorim, A.; Maio, A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.; Amorim, A.; Maio, A.] Univ Granada, CAFPE, Granada, Spain. [Bohm, J.; Chudoba, J.; Gallus, P.; Gunther, J.; Jakoubek, T.; Juranek, V.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Marcisovsky, M.; Mikestikova, M.; Myska, M.; Nemecek, S.; Ruzicka, P.; Schovancova, J.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Tic, T.; Valenta, J.; Vrba, V.; Zeman, M.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Kodys, P.; Leitner, R.; Novakova, J.; Rybar, M.; Spousta, M.; Strachota, P.; Suk, M.; Sykora, T.; Tas, P.; Valkar, S.; Vorobel, V.; Wilhelm, I.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Augsten, K.; Holy, T.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Kral, V.; Krejci, F.; Pospisil, S.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solar, M.; Solc, J.; Sopko, V.; Sopko, B.; Stekl, I.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Ammosov, V. V.; Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Ivashin, A. V.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.; Zmouchko, V. V.] Inst High Energy Phys, State Res Ctr, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Gillman, A. R.; Haywood, S. J.; Kirk, J.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Norton, P. R.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Strube, J.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Benslama, K.; Ybeles Smit, G. V.] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Shiga, Japan. [Anulli, F.; Artoni, G.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Pedis, D.; De Salvo, A.; De Zorzi, G.; Dionisi, C.; Falciano, S.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rosati, S.; Rossi, E.; Tehrani, F. Safai; Sidoti, A.; Solfaroli Camillocci, E.; Varia, R.; Veneziano, S.; Zanelloa, L.] Ist Nazl Fis Nucl, Sez Roma 1, Rome, Italy. [Artoni, G.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Zorzi, G.; Dionisi, C.; Zanelloa, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Di Simone, A.; Liberti, B.; Marchese, F.; Mazzaferro, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Cattani, G.; Di Ciaccio, A.; Di Simone, A.; Marchese, F.; Mazzaferro, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Branchini, P.; Ceradini, F.; Di Luise, S.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Soualah, R.; Stanescua, C.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Luise, S.; Orestano, D.; Pastore, F.; Petrucci, F.] Univ Roma Tre, Dipartimento Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.; Lablak, S.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA Marrakech, Fac Sci Semlalia, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Abreu, H.; Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Bolnet, N. M.; Boonekamp, M.; Chevalier, L.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Gauthier, L.; Giraud, P. F.; Guyot, C.; Hassani, S.; Hawkins, D.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Legendre, M.; Maiani, C.; Mal, P.; Ramos, J. A. Manjarres; Mansoulie, B.; Meyer, J-P.; Mijovic, L.; Morange, N.; Nguyen Thi Hong, V.; Nicolaidou, R.; Ouraou, A.; Resende, B.; Royon, C. R.; Schune, Ph.; Schwindling, J.; Simard, O.; Virchaux, M.; Vranjes, N.; Xiao, M.] CEA Saclay, DSM IRFU, Inst Rech Lois Fondamentales Univers, F-91191 Gif Sur Yvette, France. [Chouridou, S.; Damiani, D. S.; Grillo, A. A.; Hare, G. A.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Mitrevski, J.; Nielsen, J.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Beckingham, M.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Keller, J. S.; Lubatti, H. J.; Rompotis, N.; Rothberg, J.; Verducci, M.; Watts, G.; Zhao, T.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Booth, C. N.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Duxfield, R.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Mayne, A.; Mcfayden, J. A.; Miyagawa, P. S.; Owen, S.; Paganis, E.; Suruliz, K.; Tovey, D. R.; Tua, A.; Xu, D.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Holder, M.; Ibragimov, I.; Rammes, M.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-5900 Siegen, Germany. [Dawe, E.; Godfrey, J.; Kvita, J.; O'Neil, D. C.; Petteni, M.; Stelzer, B.; Tanasijczuk, A. J.; Trottier-McDonald, M.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Butler, B.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Grenier, P.; Haas, A.; Hansson, P.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nelson, T. K.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Smith, D.; Strauss, E.; Su, D.; Wilson, M. G.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Batkova, L.; Blazek, T.; Federic, P.; Pecsy, M.; Stavina, P.; Sykora, I.; Tokara, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Ferencei, J.; Kladiva, E.; Seman, M.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Aurousseau, M.; Yacooba, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Hamilton, A.; Leney, K. J. C.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Asman, B.; Bendtz, K.; Bohm, C.; Clement, C.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Holmgren, S. O.; Johansen, M.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Papadelis, A.; Sellden, B.; Silverstein, S. B.; Sjolina, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Asman, B.; Bendtz, K.; Clement, C.; Hellman, S.; Johansen, M.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Sjolina, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Ahmad, A.; Arfaoui, S.; Devetak, E.; DeWilde, B.; Engelmann, R.; Farley, J.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Dept Phys, Stony Brook, NY 11794 USA. [Ahmad, A.; Arfaoui, S.; Devetak, E.; DeWilde, B.; Engelmann, R.; Farley, J.; Hobbs, J.; Jia, J.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Bartsch, V.; De Santo, A.; Martin-Haugh, S.; Potter, C. J.; Rose, A.; Salvatore, F.; Sutton, M. R.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Bangert, A.; Cuthbert, C.; Patel, N.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Waugh, A. T.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Chu, M. L.; Hou, S.; Lee, S. C.; Lin, S. C.; Liu, D.; Mazini, R.; Meng, Z.; Ren, Z. L.; Soh, D. A.; Teng, P. K.; Wang, J.; Wang, S. M.; Weng, Z.; Zhou, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Harpaz, S. Behar; Kajomovitz, E.; Rozen, Y.; Tarem, S.; Vallecorsa, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Bella, G.; Benary, O.; Benhammou, Y.; Etzion, E.; Fournier, D.; Gershon, A.; Ginzburg, J.; Guttman, N.; Hod, N.; Munwes, Y.; Oren, Y.; Reinherz-Aronis, E.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Iliadis, D.; Kordas, K.; Kouskoura, V.; Nomidis, I.; Petridis, A.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, K.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yamazaki, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, K.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yamazaki, T.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Ishitsuka, M.; Jinnouchi, O.; Kanno, T.; Kuze, M.; Nagai, R.; Nobe, T.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Bailey, D. C.; Bain, T.; Brelier, B.; Cheung, S. L.; Dhaliwal, S.; Farooque, T.; Fatholahzadeh, B.; Gibson, A.; Guo, B.; Ilic, N.; Keung, J.; Knecht, N. S.; Krieger, P.; Le Maner, C.; Martens, F. K.; Orr, R. S.; Rezvani, R.; Rosenbaum, G. A.; Savard, P.; Schultz-Coulon, H. -C.; Sinervo, P.; Spreitzer, T.; Tardif, D.; Teuscherk, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Garcia, J. A. Benitez; Canepa, A.; Chekulaev, S. V.; Fortin, D.; Koutsman, A.; Losty, M. J.; Nugent, I. M.; Oram, C. J.; Palacino, G.; Perez Codina, E.; Schouten, D.; Stelzer-Chilton, O.; Tafirouta, R.; Taylor, W.; Triggera, I. M.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hanawa, K.; Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Kurata, M.; Nagai, K.; Ukegawa, F.] Univ Tsukuba, Inst Pure & Appl Sci, Tsukuba, Ibaraki 3058571, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Napier, A.; Rolli, S.; Sliwa, K.; Todorova-Nova, S.; Wetter, J.] Tufts Univ, Ctr Sci & Technol, Medford, MA 02155 USA. [Losada, M.; Loureiro, K. F.; Navas, L. Mendoza; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Avolio, G.; Deng, J.; Farrell, S.; Eschrich, I. Gough; Lankford, A. J.; Magnoni, L.; Mete, A. S.; Nelson, A.; Scannicchio, D. A.; Schernau, M.; Taffard, A.; Toggerson, B.; Unel, G.; Werth, M.; Wheeler-Ellis, S. J.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Del Papa, C.; Pinamonti, M.; Shaw, K.; Soualah, R.] Ist Nazl Fis Nucl, Grp Collegato Udine, Trieste, Italy. [Acharya, B. S.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Del Papa, C.; Giordani, M. P.; Pinamonti, M.; Shaw, K.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Coggeshall, J.; Cortes-Gonzalez, A.; Errede, D.; Errede, S.; Lie, K.; Liss, T. M.; McCarn, A.; Neubauer, M. S.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Brenner, R.; Buszello, C. P.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Pelikan, D.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garc, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Garcia, C.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Garc, C.; de la Hoz, S. Gonzalez; Garcia, C.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Garc, C.; de la Hoz, S. Gonzalez; Garcia, C.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Garc, C.; de la Hoz, S. Gonzalez; Garcia, C.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Axen, D.; Gay, C.; Gecse, Z.; Loh, C. W.; Mills, W. J.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Garc, C.; de la Hoz, S. Gonzalez; Garcia, C.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Llacer, M. Moreno; Garcia, E. Oliver; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; Villaplana Perez, M.; Vos, M.] CSIC, Valencia, Spain. [Albert, J.; Astbury, A.; Bansal, V.; Berghaus, F.; Courneyea, L.; Fincke-Keeler, M.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Lessard, J-R.; Marino, C. P.; Martyniuk, A. C.; McPherson, R. A.; Ouellette, E. A.; Plamondon, M.; Sobie, R.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Farrington, S. M.; Jones, G.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Kimura, N.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Alon, R.; Barak, L.; Bressler, S.; Duchovni, E.; Frank, T.; Gabizon, O.; Gross, E.; Groth-Jensen, J.; Klier, A.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Milstein, D.; Roth, I.; Silbert, O.; Smakhtin, V.; Vitells, O.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Asfandiyarov, R.; Banerjee, Sw.; Montoya, G. D. Carrillo; Hernandez, A. M. Castaneda; Castaneda-Miranda, E.; Chen, X.; Di Mattia, A.; Dos Anjos, A.; Fang, Y.; Castillo, L. R. Flores; Gonzalez, S.; Gutzwiller, O.; Ji, H.; Ju, X.; Kashif, L.; Li, H.; Ma, L. L.; Mellado Garcia, B. R.; Ming, Y.; Pan, Y. B.; Pedraza Morales, M. I.; Quayle, W. B.; Sarangi, T.; Wang, H.; Wiedenmann, W.; Wu, S. L.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Fleischmann, P.; Meyer, J.; Redelbach, A.; Siragusa, G.; Strohmer, R.; Trefzger, T.] Univ Wurzburg, Fak Phys & Astron, Wurzburg, Germany. [Barisonzi, M.; Becker, A. K.; Becks, K. H.; Boek, J.; Braun, H. M.; Cornelissen, T.; Duda, D.; Fleischmann, S.; Flick, T.; Gerlach, P.; Glitza, K. W.; Gorfine, G.; Hamacher, K.; Harenberg, T.; Henss, T.; Hirschbuehl, D.; Kalinin, S.; Kersten, S.; Khoroshilov, A.; Kohlmann, S.; Lantzsch, K.; Lenzen, G.; Mattig, P.; Mechtel, M.; Neumann, M.; Pataraia, S.; Sandhoff, M.; Sartisohn, G.; Schultes, J.; Sturm, P.; Voss, T. T.; Wagner, W.; Wahlen, H.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany. [Adelman, J.; Baker, O. K.; Bedikian, S.; Almenar, C. Cuenca; Czyczula, Z.; Demers, S.; Garberson, F.; Golling, T.; Guest, D.; Lee, L.; Loginov, A.; Sherman, D.; Tipton, P.; Wall, R.; Walsh, B.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Biscarat, C.; Cogneras, E.; Rahal, G.] Ctr Calcul CNRS IN2P3, Domaine Sci Doua, Villeurbanne, France. Univ Lisbon, Fac Ciencias, P-1699 Lisbon, Portugal. Univ Lisbon, CFNUL, P-1699 Lisbon, Portugal. Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. TRIUMF, Vancouver, BC V6T 2A3, Canada. Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. Novosibirsk State Univ, Novosibirsk 630090, Russia. Fermilab Natl Accelerator Lab, Batavia, IL USA. Univ Coimbra, Dept Phys, Coimbra, Portugal. UASLP, Dept Phys, San Luis Potosi, Mexico. Univ Napoli Parthenope, Naples, Italy. Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. Louisiana Tech Univ, Ruston, LA 71270 USA. [Wemans, A. Do Valle] Univ Nova Lisboa, Dep Fis, Caparica, Portugal. [Wemans, A. Do Valle] Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, Caparica, Portugal. UCL, Dept Phys & Astron, London, England. Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. Azerbaijan Acad Sci, Inst Phys, Baku 370143, Azerbaijan. Univ Hamburg, Inst Expt Phys, Hamburg, Germany. Manhattan Coll, New York, NY USA. Aix Marseille Univ, CPPM, Marseille, France. CNRS, IN2P3, Marseille, France. Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou, Peoples R China. Acad Sinica, Acad Sinica Grid Comp, Inst Phys, Taipei 115, Taiwan. Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. CEA Saclay, DSM IRFU, Inst Rech Lois Fondamentales Univers, F-91191 Gif Sur Yvette, France. [Nessi, M.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Pasztor, G.; Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Perez, K.] CALTECH, Pasadena, CA 91125 USA. [Richter-Was, E.] Jagiellonian Univ, Inst Phys, Krakow, Poland. [Ruan, X.] Univ Paris 11, LAL, Orsay, France. [Ruan, X.] CNRS, IN2P3, F-91405 Orsay, France. [Yacooba, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. RP Aad, G (reprint author), Univ Adelaide, Sch Chem & Phys, N Terrace Campus, Adelaide, SA 5000, Australia. RI Juste, Aurelio/I-2531-2015; Maneira, Jose/D-8486-2011; Gauzzi, Paolo/D-2615-2009; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Martinez, Mario /I-3549-2015; Monzani, Simone/D-6328-2017; Fullana Torregrosa, Esteban/A-7305-2016; Guo, Jun/O-5202-2015; Smirnova, Oxana/A-4401-2013; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Olshevskiy, Alexander/I-1580-2016; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Mora Herrera, Maria Clemencia/L-3893-2016; spagnolo, stefania/A-6359-2012; Shmeleva, Alevtina/M-6199-2015; Camarri, Paolo/M-7979-2015; Gavrilenko, Igor/M-8260-2015; Tikhomirov, Vladimir/M-6194-2015; Chekulaev, Sergey/O-1145-2015; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; Carvalho, Joao/M-4060-2013; Mashinistov, Ruslan/M-8356-2015; Booth, Christopher/B-5263-2016; Gonzalez de la Hoz, Santiago/E-2494-2016; Grinstein, Sebastian/N-3988-2014; Livan, Michele/D-7531-2012; Mitsou, Vasiliki/D-1967-2009; Joergensen, Morten/E-6847-2015; Riu, Imma/L-7385-2014; Mir, Lluisa-Maria/G-7212-2015; Garcia, Jose /H-6339-2015; Della Pietra, Massimo/J-5008-2012; Cavalli-Sforza, Matteo/H-7102-2015; Ferrer, Antonio/H-2942-2015; Prokoshin, Fedor/E-2795-2012; Hansen, John/B-9058-2015; Grancagnolo, Sergio/J-3957-2015; Mikestikova, Marcela/H-1996-2014; Kuday, Sinan/C-8528-2014; Snesarev, Andrey/H-5090-2013; Svatos, Michal/G-8437-2014; Chudoba, Jiri/G-7737-2014; Veneziano, Stefano/J-1610-2012; Peleganchuk, Sergey/J-6722-2014; Santamarina Rios, Cibran/K-4686-2014; Bosman, Martine/J-9917-2014; Lei, Xiaowen/O-4348-2014; Demirkoz, Bilge/C-8179-2014; Ventura, Andrea/A-9544-2015; Sukharev, Andrey/A-6470-2014; O'Shea, Val/G-1279-2010; Lee, Jason/B-9701-2014; Robson, Aidan/G-1087-2011; Negrini, Matteo/C-8906-2014; Fabbri, Laura/H-3442-2012; Villa, Mauro/C-9883-2009; Kepka, Oldrich/G-6375-2014; Nemecek, Stanislav/G-5931-2014; Jakoubek, Tomas/G-8644-2014; Lokajicek, Milos/G-7800-2014; Staroba, Pavel/G-8850-2014; Kupco, Alexander/G-9713-2014; Conde Muino, Patricia/F-7696-2011; Andreazza, Attilio/E-5642-2011; Boyko, Igor/J-3659-2013; Kuleshov, Sergey/D-9940-2013; Anjos, Nuno/I-3918-2013; Kartvelishvili, Vakhtang/K-2312-2013; Dawson, Ian/K-6090-2013; Marti-Garcia, Salvador/F-3085-2011; Wolters, Helmut/M-4154-2013; Warburton, Andreas/N-8028-2013; De, Kaushik/N-1953-2013; Stoicea, Gabriel/B-6717-2011; Brooks, William/C-8636-2013; Doyle, Anthony/C-5889-2009; Pina, Joao /C-4391-2012; Amorim, Antonio/C-8460-2013; Solfaroli Camillocci, Elena/J-1596-2012; Vanyashin, Aleksandr/H-7796-2013; Ferrando, James/A-9192-2012; Casadei, Diego/I-1785-2013; La Rosa, Alessandro/I-1856-2013; Moraes, Arthur/F-6478-2010; Smirnov, Sergei/F-1014-2011; Petrucci, Fabrizio/G-8348-2012; Annovi, Alberto/G-6028-2012; Fazio, Salvatore /G-5156-2010; Bergeaas Kuutmann, Elin/A-5204-2013; Wemans, Andre/A-6738-2012; Cascella, Michele/B-6156-2013; Alexa, Calin/F-6345-2010; messina, andrea/C-2753-2013; Weigell, Philipp/I-9356-2012; de Groot, Nicolo/A-2675-2009; Moorhead, Gareth/B-6634-2009; Ma, Hong/F-2725-2011; Orlov, Ilya/E-6611-2012; OI Dell'Asta, Lidia/0000-0002-9601-4225; abi, babak/0000-0001-7036-9645; Chen, Hucheng/0000-0002-9936-0115; Cataldi, Gabriella/0000-0001-8066-7718; Sawyer, Lee/0000-0001-8295-0605; Turra, Ruggero/0000-0001-8740-796X; Anjos, Nuno/0000-0002-0018-0633; Juste, Aurelio/0000-0002-1558-3291; Begel, Michael/0000-0002-1634-4399; Thomson, Mark/0000-0002-2654-9005; Vari, Riccardo/0000-0002-2814-1337; Nisati, Aleandro/0000-0002-5080-2293; Maneira, Jose/0000-0002-3222-2738; Gauzzi, Paolo/0000-0003-4841-5822; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Monzani, Simone/0000-0002-0479-2207; Troncon, Clara/0000-0002-7997-8524; Bailey, David C/0000-0002-7970-7839; Fullana Torregrosa, Esteban/0000-0003-3082-621X; Gray, Heather/0000-0002-5293-4716; Abdelalim, Ahmed Ali/0000-0002-2056-7894; Nielsen, Jason/0000-0002-9175-4419; Guo, Jun/0000-0001-8125-9433; Smirnova, Oxana/0000-0003-2517-531X; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Olshevskiy, Alexander/0000-0002-8902-1793; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; spagnolo, stefania/0000-0001-7482-6348; Camarri, Paolo/0000-0002-5732-5645; Tikhomirov, Vladimir/0000-0002-9634-0581; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; Carvalho, Joao/0000-0002-3015-7821; Mashinistov, Ruslan/0000-0001-7925-4676; Booth, Christopher/0000-0002-6051-2847; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Cranmer, Kyle/0000-0002-5769-7094; Mincer, Allen/0000-0002-6307-1418; Grinstein, Sebastian/0000-0002-6460-8694; Amorim, Antonio/0000-0003-0638-2321; Evans, Harold/0000-0003-2183-3127; Cristinziani, Markus/0000-0003-3893-9171; Chromek-Burckhart, Doris/0000-0003-4243-3288; Qian, Jianming/0000-0003-4813-8167; Livan, Michele/0000-0002-5877-0062; Mitsou, Vasiliki/0000-0002-1533-8886; Joergensen, Morten/0000-0002-6790-9361; Riu, Imma/0000-0002-3742-4582; Mir, Lluisa-Maria/0000-0002-4276-715X; Della Pietra, Massimo/0000-0003-4446-3368; Ferrer, Antonio/0000-0003-0532-711X; Prokoshin, Fedor/0000-0001-6389-5399; Hansen, John/0000-0002-8422-5543; Grancagnolo, Sergio/0000-0001-8490-8304; Mikestikova, Marcela/0000-0003-1277-2596; Kuday, Sinan/0000-0002-0116-5494; Svatos, Michal/0000-0002-7199-3383; Veneziano, Stefano/0000-0002-2598-2659; Peleganchuk, Sergey/0000-0003-0907-7592; Santamarina Rios, Cibran/0000-0002-9810-1816; Bosman, Martine/0000-0002-7290-643X; Lei, Xiaowen/0000-0002-2564-8351; Ventura, Andrea/0000-0002-3368-3413; O'Shea, Val/0000-0001-7183-1205; Lee, Jason/0000-0002-2153-1519; Negrini, Matteo/0000-0003-0101-6963; Fabbri, Laura/0000-0002-4002-8353; Villa, Mauro/0000-0002-9181-8048; Conde Muino, Patricia/0000-0002-9187-7478; Andreazza, Attilio/0000-0001-5161-5759; Boyko, Igor/0000-0002-3355-4662; Kuleshov, Sergey/0000-0002-3065-326X; Wolters, Helmut/0000-0002-9588-1773; Warburton, Andreas/0000-0002-2298-7315; De, Kaushik/0000-0002-5647-4489; Stoicea, Gabriel/0000-0002-7511-4614; Brooks, William/0000-0001-6161-3570; Doyle, Anthony/0000-0001-6322-6195; Pina, Joao /0000-0001-8959-5044; Solfaroli Camillocci, Elena/0000-0002-5347-7764; Vanyashin, Aleksandr/0000-0002-0367-5666; Ferrando, James/0000-0002-1007-7816; La Rosa, Alessandro/0000-0001-6291-2142; Moraes, Arthur/0000-0002-5157-5686; Smirnov, Sergei/0000-0002-6778-073X; Petrucci, Fabrizio/0000-0002-5278-2206; Annovi, Alberto/0000-0002-4649-4398; Wemans, Andre/0000-0002-9669-9500; Cascella, Michele/0000-0003-2091-2501; Moorhead, Gareth/0000-0002-9299-9549; Orlov, Ilya/0000-0003-4073-0326; Haas, Andrew/0000-0002-4832-0455; Vos, Marcel/0000-0001-8474-5357; Castro, Nuno/0000-0001-8491-4376; Hays, Chris/0000-0003-2371-9723; Farrington, Sinead/0000-0001-5350-9271; Filthaut, Frank/0000-0003-3338-2247; Belanger-Champagne, Camille/0000-0003-2368-2617; Robson, Aidan/0000-0002-1659-8284; Weber, Michele/0000-0002-2770-9031; Strube, Jan/0000-0001-7470-9301; Beck, Hans Peter/0000-0001-7212-1096; Prokofiev, Kirill/0000-0002-2177-6401; Vazquez Schroeder, Tamara/0000-0002-9780-099X; Chen, Chunhui /0000-0003-1589-9955; Walsh, Brian/0000-0003-1689-2309 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union; ERC, European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; ISF, Israel; MINERVA, Israel; GIF, Israel; DIP, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; GRICES, Portugal; FCT, Portugal; MERYS (MECTS), Romania; MES of Russia, Russian Federation; ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MVZT, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET and ERC, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT, Greece; ISF, MINERVA, GIF, DIP and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW, Poland; GRICES and FCT, Portugal; MERYS (MECTS), Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MVZT, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. NR 80 TC 9 Z9 9 U1 4 U2 108 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD NOV PY 2012 IS 11 AR 094 DI 10.1007/JHEP11(2012)094 PG 35 WC Physics, Particles & Fields SC Physics GA 052LG UT WOS:000312198500029 ER PT J AU Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hammer, J Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Liko, D Mikulec, I Pernicka, M Rahbaran, B Rohringer, C Rohringer, H Schofbeck, R Strauss, J Taurok, A Wagner, P Waltenberger, W Walzel, G Widl, E Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Bansal, S Cornelis, T De Wolf, EA Janssen, X Luyckx, S Maes, T Mucibello, L Ochesanu, S Roland, B Rougny, R Selvaggi, M Staykova, Z Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Suarez, RG Kalogeropoulos, A Maes, M Olbrechts, A Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Clerbaux, B De Lentdecker, G Dero, V Gay, APR Hreus, T Leonard, A Marage, PE Reis, T Thomas, L Vander Velde, C Vanlaer, P Wang, J Adler, V Beernaert, K Cimmino, A Costantini, S Garcia, G Grunewald, M Klein, B Lellouch, J Marinov, A Mccartin, J Rios, AAO Ryckbosch, D Strobbe, N Thyssen, F Tytgat, M Vanelderen, L Verwilligen, P Walsh, S Yazgan, E Zaganidis, N Basegmez, S Bruno, G Castello, R Caudron, A Ceard, L Delaere, C du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Lemaitre, V Liao, J Militaru, O Nuttens, C Pagano, D Perrini, L Pin, A Piotrzkowski, K Schul, N Garcia, JMV Beliy, N Caebergs, T Daubie, E Hammad, GH Alves, GA Martins, MC Damiao, DDJ Martins, T Pol, ME Souza, MHG Alda, WL Carvalho, W Custodio, A Da Costa, EM Martins, CD De Souza, SF Figueiredo, DM Mundim, L Nogima, H Oguri, V Da Silva, WLP Santoro, A Jorge, LS Sznajder, A Bernardes, CA Dias, FA Tomei, TRFP Gregores, EM Lagana, C Marinho, F Mercadante, PG Novaes, SF Padula, SS Genchev, V Iaydjiev, P Piperov, S Rodozov, M Stoykova, S Sultanov, G Tcholakov, V Trayanov, R Vutova, M Dimitrov, A Hadjiiska, R Kozhuharov, V Litov, L Pavlov, B Petkov, P Bian, JG Chen, GM Chen, HS Jiang, CH Liang, D Liang, S Meng, X Tao, J Wang, J Wang, X Wang, Z Xiao, H Xu, M Zang, J Zhang, Z Asawatangtrakuldee, C Ban, Y Guo, S Guo, Y Li, W Liu, S Mao, Y Qian, SJ Teng, H Wang, S Zhu, B Zou, W Avila, C Gomez, JP Moreno, BG Oliveros, AFO Sanabria, JC Godinovic, N Lelas, D Plestina, R Polic, D Puljak, I Antunovic, Z Kovac, M Brigljevic, V Duric, S Kadija, K Luetic, J Morovic, S Attikis, A Galanti, M Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Finger, M Finger, M Assran, Y Elgammal, S Kamel, AE Khalil, S Mahmoud, MA Radi, A Kadastik, M Muntel, M Raidal, M Rebane, L Tiko, A Azzolini, V Eerola, P Fedi, G Voutilainen, M Hakonen, J Heikkinen, A Karimaki, V Kinnunen, R Kortelainen, MJ Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E Ungaro, D Wendland, L Banzuzi, K Karjalainen, A Korpela, A Tuuva, T Besancon, M Choudhury, S Dejardin, M Denegri, D Fabbro, B Faure, JL Ferri, F Ganjour, S Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Malcles, J Millischer, L Nayak, A Rander, J Rosowsky, A Shreyber, I Titov, M Baffioni, S Beaudette, F Benhabib, L Bianchini, L Bluj, M Broutin, C Busson, P Charlot, C Daci, N Dahms, T Dobrzynski, L de Cassagnac, RG Haguenauer, M Mine, P Mironov, C Nguyen, M Ochando, C Paganini, P Sabes, D Salerno, R Sirois, Y Veelken, C Zabi, A Agram, JL Andrea, J Bloch, D Bodin, D Brom, JM Cardaci, M Chabert, EC Collard, C Conte, E Drouhin, F Ferro, C Fontaine, JC Gele, D Goerlach, U Juillot, P Le Bihan, AC Van Hove, P Fassi, F Mercier, D Beauceron, S Beaupere, N Bondu, O Boudoul, G Chasserat, J Chierici, R Contardo, D Depasse, P El Mamouni, H Fay, J Gascon, S Gouzevitch, M Ille, B Kurca, T Lethuillier, M Mirabito, L Perries, S Sordini, V Tosi, S Tschudi, Y Verdier, P Viret, S Tsamalaidze, Z Anagnostou, G Beranek, S Edelhoff, M Feld, L Heracleous, N Hindrichs, O Jussen, R Klein, K Merz, J Ostapchuk, A Perieanu, A Raupach, F Sammet, J Schael, S Sprenger, D Weber, H Wittmer, B Zhukov, V Ata, M Caudron, J Dietz-Laursonn, E Duchardt, D Erdmann, M Fischer, R Guth, A Hebbeker, T Heidemann, C Hoepfner, K Klingebiel, D Kreuzer, P Lingemann, J Magass, C Merschmeyer, M Meyer, A Olschewski, M Papacz, P Pieta, H Reithler, H Schmitz, SA Sonnenschein, L Steggemann, J Teyssier, D Weber, M Bontenackels, M Cherepanov, V Flugge, G Geenen, H Geisler, M Ahmad, WH Hoehle, F Kargoll, B Kress, T Kuessel, Y Nowack, A Perchalla, L Pooth, O Rennefeld, J Sauerland, P Stahl, A Martin, MA Behr, J Behrenhoff, W Behrens, U Bergholz, M Bethani, A Borras, K Burgmeier, A Cakir, A Calligaris, L Campbell, A Castro, E Costanza, F Dammann, D Pardos, CD Eckerlin, G Eckstein, D Flucke, G Geiser, A Glushkov, I Gunnellini, P Habib, S Hauk, J Hellwig, G Jung, H Kasemann, M Katsas, P Kleinwort, C Kluge, H Knutsson, A Kramer, M Krucker, D Kuznetsova, E Lange, W Lohmann, W Lutz, B Mankel, R Marfin, I Marienfeld, M Melzer-Pellmann, IA Meyer, AB Mnich, J Mussgiller, A Naumann-Emme, S Olzem, J Perrey, H Petrukhin, A Pitzl, D Raspereza, A Cipriano, PMR Riedl, C Ron, E Rosin, M Salfeld-Nebgen, J Schmidt, R Schoerner-Sadenius, T Sen, N Spiridonov, A Stein, M Walsh, R Wissing, C Autermann, C Blobel, V Bobrovskyi, S Draeger, J Enderle, H Erfle, J Gebbert, U Gorner, M Hermanns, T Hoing, RS Kaschube, K Kaussen, G Kirschenmann, H Klanner, R Lange, J Mura, B Nowak, F Peiffer, T Pietsch, N Rathjens, D Sander, C Schettler, H Schleper, P Schlieckau, E Schmidt, A Schroder, M Schum, T Seidel, M Stadie, H Steinbruck, G Thomsen, J Barth, C Berger, J Boser, C Chwalek, T De Boer, W Descroix, A Dierlamm, A Feindt, M Guthoff, M Hackstein, C Hartmann, F Hauth, T Heinrich, M Held, H Hoffmann, KH Honc, S Katkov, I Komaragiri, JR Martschei, D Mueller, S Muller, T Niegel, M Nurnberg, A Oberst, O Oehler, A Ott, J Quast, G Rabbertz, K Ratnikov, F Ratnikova, N Rocker, S Scheurer, A Schilling, FP Schott, G Simonis, HJ Stober, FM Troendle, D Ulrich, R Wagner-Kuhr, J Wayand, S Weiler, T Zeise, M Daskalakis, G Geralis, T Kesisoglou, S Kyriakis, A Loukas, D Manolakos, I Markou, A Markou, C Mavrommatis, C Ntomari, E Gouskos, L Mertzimekis, TJ Panagiotou, A Saoulidou, N Evangelou, I Foudas, C Kokkas, P Manthos, N Papadopoulos, I Patras, V Bencze, G Hajdu, C Hidas, P Horvath, D Sikler, F Veszpremi, V Vesztergombi, G Beni, N Czellar, S Molnar, J Palinkas, J Szillasi, Z Karancsi, J Raics, P Trocsanyi, ZL Ujvari, B Bansal, M Beri, SB Bhatnagar, V Dhingra, N Gupta, R Kaur, M Mehta, MZ Nishu, N Saini, LK Sharma, A Singh, JB Kumar, A Kumar, A Ahuja, S Bhardwaj, A Choudhary, BC Malhotra, S Naimuddin, M Ranjan, K Sharma, V Shivpuri, RK Banerjee, S Bhattacharya, S Dutta, S Gomber, B Jain, S Jain, S Khurana, R Sarkar, S Sharan, M Abdulsalam, A Choudhury, RK Dutta, D Kailas, S Kumar, V Mehta, P Mohanty, AK Pant, LM Shukla, P Aziz, T Ganguly, S Guchait, M Maity, M Majumder, G Mazumdar, K Mohanty, GB Parida, B Sudhakar, K 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Choi, YK Goh, J Kim, MS Kwon, E Lee, B Lee, J Lee, S Seo, H Yu, I Bilinskas, MJ Grigelionis, I Janulis, M Juodagalvis, A Castilla-Valdez, H De La Cruz-Burelo, E Heredia-de La Cruz, I Lopez-Fernandez, R Villalba, RM Martinez-Ortega, J Sanchez-Hernandez, A Villasenor-Cendejas, LM Moreno, SC Valencia, FV Ibarguen, HA Linares, EC Pineda, AM Reyes-Santos, MA Krofcheck, D Bell, AJ Butler, PH Doesburg, R Reucroft, S Silverwood, H Ahmad, M Asghar, MI Hoorani, HR Khalid, S Khan, WA Khurshid, T Qazi, S Shah, MA Shoaib, M Bialkowska, H Boimska, B Frueboes, T Gokieli, R Gorski, M Kazana, M Nawrocki, K Romanowska-Rybinska, K Szleper, M Wrochna, G Zalewski, P Brona, G Bunkowski, K Cwiok, M Dominik, W Doroba, K Kalinowski, A Konecki, M Krolikowski, J Almeida, N Bargassa, P David, A Faccioli, P Fernandes, M Parracho, PGF Gallinaro, M Seixas, J Varela, J Vischia, P Belotelov, I Bunin, P Gavrilenko, M Golutvin, I Gorbunov, I Kamenev, A Karjavin, V Kozlov, G Lanev, A Malakhov, A Moisenz, P Palichik, V Perelygin, V Shmatov, S Smirnov, V Volodko, A Zarubin, A Evstyukhin, S Golovtsov, V Ivanov, Y Kim, V Levchenko, P Murzin, V Oreshkin, V Smirnov, I Sulimov, V Uvarov, L Vavilov, S Vorobyev, A Vorobyev, A Andreev, Y Dermenev, A Gninenko, S Golubev, N Kirsanov, M Krasnikov, N Matveev, V Pashenkov, A Tlisov, D Toropin, A Epshteyn, V Erofeeva, M Gavrilov, V Kossov, M Lychkovskaya, N Popov, V Safronov, G Semenov, S Stolin, V Vlasov, E Zhokin, A Belyaev, A Boos, E Dudko, L Ershov, A Gribushin, A Khein, L Klyukhin, V Kodolova, O Markina, A Obraztsov, S Perfilov, M Petrushanko, S Popov, A Proskuryakov, A Sarycheva, L Savrin, V Andreev, V Azarkin, M Dremin, I Kirakosyan, M Leonidov, A Mesyats, G Rusakov, SV Vinogradov, A Azhgirey, I Bayshev, I Bitioukov, S Grishin, V Kachanov, V Konstantinov, D Korablev, A Krychkine, V Petrov, V Ryutin, R Sobol, A Tourtchanovitch, L Troshin, S Tyurin, N Uzunian, A Volkov, A Adzic, P Djordjevic, M Ekmedzic, M Krpic, D Milosevic, J Aguilar-Benitez, M Maestre, JA Arce, P Battilana, C Calvo, E Cerrada, M Llatas, M Colino, N De La Cruz, B Peris, AD Vazquez, DD Bedoya, C Ramos, JPF Ferrando, A Flix, J Fouz, MC Garcia-Abia, P Lopez, OG Lopez, SG Hernandez, JM Josa, MI Merino, G Pelayo, JP Olmeda, AQ Redondo, I Romero, L Santaolalla, J Soares, MS Willmott, C Albajar, C Codispoti, G de Troconiz, JF Brun, H Cuevas, J Menendez, JF Folgueras, S Caballero, IG Iglesias, LL Gomez, JP Cifuentes, JAB Cabrillo, IJ Calderon, A Chuang, SH Campderros, JD Felcini, M Fernandez, M Gomez, G Sanchez, JG Jorda, C Pardo, PL Virto, AL Marco, J Marco, R Rivero, CM Matorras, F Sanchez, FJM Rodrigo, T Rodriguez-Marrero, AY Ruiz-Jimeno, A Scodellaro, L Sanudo, MS Vila, I Cortabitarte, RV Abbaneo, D Auffray, E Auzinger, G Baillon, P Ball, AH Barney, D Bernet, C Bianchi, G Bloch, P Bocci, A Bonato, A Botta, C Breuker, H Camporesi, T Cerminara, G Christiansen, T Perez, JAC D'Enterria, D Dabrowski, A De Roeck, A Di Guida, S Dobson, M Dupont-Sagorin, N Elliott-Peisert, A Frisch, 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Baeni, L Bortignon, P Buchmann, MA Casal, B Chanon, N Deisher, A Dissertori, G Dittmar, M Duenser, M Eugster, J Freudenreich, K Grab, C Hits, D Lecomte, P Lustermann, W Marini, AC del Arbol, PMR Mohr, N Moortgat, F Naegeli, C Nef, P Nessi-Tedaldi, F Pandolfi, F Pape, L Pauss, F Peruzzi, M Ronga, FJ Rossini, M Sala, L Sanchez, AK Starodumov, A Stieger, B Takahashi, M Tauscher, L Thea, A Theofilatos, K Treille, D Urscheler, C Wallny, R Weber, HA Wehrli, L Aguilo, E Amsler, C Chiochia, V De Visscher, S Favaro, C Rikova, MI Mejias, BM Otiougova, P Robmann, P Snoek, H Tupputi, S Verzetti, M Chang, YH Chen, KH Kuo, CM Li, SW Lin, W Liu, ZK Lu, YJ Mekterovic, D Singh, AP Volpe, R Yu, SS Bartalini, P Chang, P Chang, YH Chang, YW Chao, Y Chen, KF Dietz, C Grundler, U Hou, WS Hsiung, Y Kao, KY Lei, YJ Lu, RS Majumder, D Petrakou, E Shi, X Shiu, JG Tzeng, YM Wan, X Wang, M Adiguzel, A Bakirci, MN Cerci, S Dozen, C Dumanoglu, I Eskut, E Girgis, S Gokbulut, G Gurpinar, E Hos, I Kangal, EE Karapinar, G Topaksu, AK Onengut, G Ozdemir, K Ozturk, S Polatoz, A Sogut, K Cerci, DS Tali, B Topakli, H Vergili, LN Vergili, M Akin, IV Aliev, T Bilin, B Bilmis, S Deniz, M Gamsizkan, H Guler, AM Ocalan, K Ozpineci, A Serin, M Sever, R Surat, UE Yalvac, M Yildirim, E Zeyrek, M Gulmez, E Isildak, B Kaya, M Kaya, O Ozkorucuklu, S Sonmez, N Cankocak, K Levchuk, L Bostock, F Brooke, JJ Clement, E Cussans, D Flacher, H Frazier, R Goldstein, J Grimes, M Heath, GP Heath, HF Kreczko, L Metson, S Newbold, DM Nirunpong, K Poll, A Senkin, S Smith, VJ Williams, T Basso, L Bell, KW Belyaev, A Brew, C Brown, RM Cockerill, DJA Coughlan, JA Harder, K Harper, S Jackson, J Kennedy, BW Olaiya, E Petyt, D Radburn-Smith, BC Shepherd-Themistocleous, CH Tomalin, IR Womersley, WJ Bainbridge, R Ball, G Beuselinck, R Buchmuller, O Colling, D Cripps, N Cutajar, M Dauncey, P Davies, G Della Negra, M Ferguson, W Fulcher, J Futyan, D Gilbert, A Bryer, AG Hall, G Hatherell, Z Hays, J Iles, G Jarvis, M Karapostoli, 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CA CMS Collaboration TI Search for exclusive or semi-exclusive gamma gamma production and observation of exclusive and semi-exclusive e(+)e(-) production in pp collisions at root s=7 TeV SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering ID DOUBLE-POMERON EXCHANGE; HADRON COLLIDERS; HIGGS PRODUCTION; LHC; DIFFRACTION; TEVATRON AB A search for exclusive or semi-exclusive gamma gamma production, pp -> p(()*()) + gamma gamma + p(()*()) (where p* stands for a diffractively-dissociated proton), and the observation of exclusive and semi-exclusive e(+)e(-) production, pp -> p(()*()) + e(+)e(-) + p(()*()), in proton-proton collisions at root s = 7 TeV, are presented. The analysis is based on a data sample corresponding to an integrated luminosity of 36 pb(-1) recorded by the CMS experiment at the LHC at low instantaneous luminosities. Candidate gamma gamma or e(+)e(-) events are selected by requiring the presence of two photons or a positron and an electron, each with transverse energy E-T > 5.5 GeV and pseudorapidity vertical bar eta vertical bar < 2.5, and no other particles in the region vertical bar eta vertical bar < 5.2. No exclusive or semi-exclusive diphoton candidates are found in the data. An upper limit on the cross section for the reaction pp -> p(()*()) + gamma gamma + p(()*()), within the above kinematic selections, is set at 1.18 pb at 95% confidence level. Seventeen exclusive or semi-exclusive dielectron candidates are observed, with an estimated background of 0.85 +/- 0.28 (stat.) events, in agreement with the QED-based prediction of 16.3 +/- 1.3 (syst.) events. C1 [Chatrchyan, S.; Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Bergauer, T.; Dragicevic, M.; Eroe, J.; Fabjan, C.; Friedl, M.; Fruehwirth, R.; Ghete, V. 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R.; Martschei, D.; Mueller, S.; Mueller, Th.; Niegel, M.; Nuernberg, A.; Oberst, O.; Oehler, A.; Ott, J.; Quast, G.; Rabbertz, K.; Ratnikov, F.; Ratnikova, N.; Roecker, S.; Scheurer, A.; Schilling, F. -P.; Schott, G.; Simonis, H. J.; Stober, F. M.; Troendle, D.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weiler, T.; Zeise, M.] Univ Karlsruhe, Inst Expt Kernphys, D-7500 Karlsruhe, Germany. [Daskalakis, G.; Geralis, T.; Kesisoglou, S.; Kyriakis, A.; Loukas, D.; Manolakos, I.; Markou, A.; Markou, C.; Mavrommatis, C.; Ntomari, E.] Inst Nucl Phys Demokritos, Aghia Paraskevi, Greece. [Gouskos, L.; Mertzimekis, T. J.; Panagiotou, A.; Saoulidou, N.] Univ Athens, Athens, Greece. [Evangelou, I.; Foudas, C.; Kokkas, P.; Manthos, N.; Papadopoulos, I.; Patras, V.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.] KFKI Res Inst Particle & Nucl Phys, Budapest, Hungary. [Beni, N.; Czellar, S.; Molnar, J.; Palinkas, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Karancsi, J.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, H-4012 Debrecen, Hungary. [Bansal, M.; Beri, S. B.; Bhatnagar, V.; Dhingra, N.; Gupta, R.; Kaur, M.; Mehta, M. Z.; Nishu, N.; Saini, L. K.; Sharma, A.; Singh, J. B.] Panjab Univ, Chandigarh 160014, India. [Kumar, Ashok; Kumar, Arun; Ahuja, S.; Bhardwaj, A.; Choudhary, B. C.; Malhotra, S.; Naimuddin, M.; Ranjan, K.; Sharma, V.; Shivpuri, R. K.] Univ Delhi, Delhi 110007, India. [Banerjee, S.; Bhattacharya, S.; Dutta, S.; Gomber, B.; Jain, Sa.; Jain, Sh.; Khurana, R.; Sarkar, S.; Sharan, M.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Choudhury, R. K.; Dutta, D.; Kailas, S.; Kumar, V.; Mehta, P.; Mohanty, A. K.; Pant, L. M.; Shukla, P.] Bhabha Atom Res Ctr, Bombay 400085, Maharashtra, India. [Aziz, T.; Ganguly, S.; Guchait, M.; Maity, M.; Majumder, G.; Mazumdar, K.; Mohanty, G. B.; Parida, B.; Sudhakar, K.; Wickramage, N.] Tata Inst Fundamental Res EHEP, Bombay, Maharashtra, India. [Arfaei, H.; Bakhshiansohi, H.; Etesami, S. M.; Fahim, A.; Hashemi, M.; Jafari, A.; Khakzad, M.; Mohammadi, A.; Najafabadi, M. Mohammadi; Mehdiabadi, S. Paktinat; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; Colaleo, A.; Creanza, D.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Lusito, L.; Maggi, G.; Maggi, M.; Marangelli, B.; My, S.; Nuzzo, S.; Pacifico, N.; Pompili, A.; Pugliese, G.; Selvaggi, G.; Silvestris, L.; Singh, G.; Zito, G.] INFN Sez Bari, Bari, Italy. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; Colaleo, A.; Creanza, D.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Lusito, L.; Maggi, G.; Maggi, M.; Marangelli, B.; My, S.; Nuzzo, S.; Pacifico, N.; Pompili, A.; Pugliese, G.; Selvaggi, G.; Silvestris, L.; Singh, G.; Venditti, R.; Zito, G.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Meneghelli, M.; Montanari, A.; Navarria, F. L.; Odorici, F.; Perrotta, A.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Travaglini, R.] INFN Sez Bologna, Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Capiluppi, P.; Castro, A.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Meneghelli, M.; Navarria, F. L.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] INFN Sez Catania, Catania, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Maity, M.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Bakhshiansohi, H.; Fahim, A.; Jafari, A.] Sharif Univ Technol, Tehran, Iran. [Etesami, S. M.; Zeinali, M.] Isfahan Univ Technol, Esfahan, Iran. [Mohammadi, A.] Shiraz Univ, Shiraz, Iran. [Safarzadeh, B.] Islamic Azad Univ, Sci & Res Branch, Plasma Phys Res Ctr, Tehran, Iran. [Colafranceschi, S.] Univ Rome, Fac Ingn, Rome, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata, I-85100 Potenza, Italy. [Meola, S.] Univ Guglielmo Marconi, Rome, Italy. [Gulmini, M.] Lab Nazl Legnaro INFN, Legnaro, Italy. [Martini, L.] Univ Siena, I-53100 Siena, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gallo, E.; Gonzi, S.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] INFN Sez Firenze, Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gonzi, S.] Univ Florence, Florence, Italy. [Fabbri, F.; Benussi, L.; Bianco, S.; Colafranceschi, S.; Piccolo, D.] INFN Lab Nazl Frascati, Frascati, Italy. [Fabbricatore, P.; Musenich, R.] INFN Sez Genova, Genoa, Italy. Univ Genoa, Genoa, Italy. [Benaglia, A.; De Guio, F.; Di Matteo, L.; Fiorendi, S.; Gennai, S.; Ghezzi, A.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Massironi, A.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; Sala, S.; de Fatis, T. Tabarelli] INFN Sez Milano Bicocca, Milan, Italy. [Benaglia, A.; De Guio, F.; Di Matteo, L.; Fiorendi, S.; Ghezzi, A.; Manzoni, R. A.; Martelli, A.; Massironi, A.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Montoya, C. A. Carrillo; Cavallo, N.; De Cosa, A.; Dogangun, O.; Fabozzi, F.; Iorio, A. O. M.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.] INFN Sez Napoli, Naples, Italy. [De Cosa, A.; Dogangun, O.; Merola, M.] Univ Naples Federico II, Naples, Italy. [Azzi, P.; Bacchetta, N.; Bisello, D.; Branca, A.; Carlin, R.; Checchia, P.; Dorigo, T.; Gasparini, F.; Gasparini, U.; Gozzelino, A.; Gulmini, M.; Kanishchev, K.; Lacaprara, S.; Lazzizzera, I.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Vanini, S.; Zotto, P.; Zucchetta, A.; Zumerle, G.] INFN Sez Padova, Padua, Italy. [Bisello, D.; Branca, A.; Carlin, R.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Vanini, S.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.; Lazzizzera, I.] Univ Trento Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Torre, P.; Vitulo, P.] INFN Sez Pavia, Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Torre, P.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Fano, L.; Lariccia, P.; Lucaroni, A.; Mantovani, G.; Menichelli, M.; Nappi, A.; Romeo, F.; Saha, A.; Santocchia, A.; Taroni, S.] INFN Sez Perugia, Perugia, Italy. [Biasini, M.; Fano, L.; Lariccia, P.; Lucaroni, A.; Mantovani, G.; Nappi, A.; Romeo, F.; Santocchia, A.; Taroni, S.] Univ Perugia, I-06100 Perugia, Italy. [Azzurri, P.; Bagliesi, G.; Boccali, T.; Broccolo, G.; Castaldi, R.; D'Agnolo, R. T.; Dell'Orso, R.; Fiori, F.; Foa, L.; Giassi, A.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] INFN Sez Pisa, Pisa, Italy. [Fiori, F.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Azzurri, P.; Broccolo, G.; D'Agnolo, R. T.; Foa, L.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Diemoz, M.; Grassi, M.; Longo, E.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Sigamani, M.; Soffi, L.] INFN Sez Roma, Rome, Italy. [Barone, L.; Del Re, D.; Grassi, M.; Longo, E.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Soffi, L.] Univ Roma La Sapienza, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Biino, C.; Cartiglia, N.; Costa, M.; Demaria, N.; Graziano, A.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Pastrone, N.; Pelliccioni, M.; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Sola, V.; Solano, A.; Staiano, A.; Pereira, A. Vilela] INFN Sez Torino, Turin, Italy. [Amapane, N.; Argiro, S.; Costa, M.; Graziano, A.; Migliore, E.; Monaco, V.; Potenza, A.; Romero, A.; Sacchi, R.; Sola, V.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; Marone, M.; Montanino, D.; Penzo, A.; Schizzi, A.] INFN Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; Marone, M.; Montanino, D.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Heo, S. G.; Kim, T. Y.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Chang, S.; Chung, J.; Kim, D. H.; Kim, G. N.; Kong, D. J.; Park, H.; Ro, S. R.; Son, D. C.; Son, T.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, J. Y.; Kim, Zero J.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, T. J.; Lee, K. S.; Moon, D. H.; Park, S. K.] Korea Univ, Seoul, South Korea. [Choi, M.; Kang, S.; Kim, J. H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Cho, Y.; Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. S.; Kwon, E.; Lee, B.; Lee, J.; Lee, S.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Bilinskas, M. J.; Grigelionis, I.; Janulis, M.; Juodagalvis, A.] Vilnius State Univ, Vilnius, Lithuania. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Lopez-Fernandez, R.; Magana Villalba, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] Ctr Invest & Estudios Avanzados IPN, Mexico City, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.; Reyes-Santos, M. A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Campbell, A.; Butler, P. H.; Doesburg, R.; Reucroft, S.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Asghar, M. I.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Boimska, B.; Frueboes, T.; Gokieli, R.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Almeida, N.; Bargassa, P.; David, A.; Faccioli, P.; Fernandes, M.; Ferreira Parracho, P. G.; Gallinaro, M.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Belotelov, I.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Kozlov, G.; Lanev, A.; Malakhov, A.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Smirnov, V.; Volodko, A.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Evstyukhin, S.; Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Krasnikov, N.; Matveev, V.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Kirakosyan, M.] Russian Acad Sci, Inst Nucl Res, Moscow, Russia. [Epshteyn, V.; Erofeeva, M.; Gavrilov, V.; Kossov, M.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Stolin, V.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Belyaev, A.; Boos, E.; Dudko, L.; Ershov, A.; Gribushin, A.; Khein, L.; Klyukhin, V.; Kodolova, O.; Markina, A.; Obraztsov, S.; Perfilov, M.; Petrushanko, S.; Popov, A.; Proskuryakov, A.; Sarycheva, L.; Savrin, V.] Moscow MV Lomonosov State Univ, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Grishin, V.; Kachanov, V.; Konstantinov, D.; Korablev, A.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Alcaraz Maestre, J.; Arce, P.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.; Willmott, C.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Chuang, S. H.; Duarte Campderros, J.; Felcini, M.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Jorda, C.; Lobelle Pardo, P.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Sobron Sanudo, M.; Vila, I.; Vilar Cortabitarte, R.] CSIC Univ Cantabria, Inst Fis Cantabria IFCA, Santander, Spain. [Bertl, W.; Deiters, K.; Erdmann, W.; Gabathuler, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Meier, F.; Renker, D.; Rohe, T.; Sibille, J.] Paul Scherrer Inst, Villigen, Switzerland. [Baeni, L.; Bortignon, P.; Buchmann, M. A.; Casal, B.; Chanon, N.; Deisher, A.; Dissertori, G.; Dittmar, M.; Duenser, M.; Eugster, J.; Freudenreich, K.; Grab, C.; Hits, D.; Lecomte, P.; Lustermann, W.; Marini, A. C.; del Arbol, P. Martinez Ruiz; Mohr, N.; Moortgat, F.; Naegeli, C.; Nef, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pape, L.; Pauss, F.; Peruzzi, M.; Ronga, F. J.; Rossini, M.; Sala, L.; Sanchez, A. K.; Starodumov, A.; Stieger, B.; Takahashi, M.; Tauscher, L.; Thea, A.; Theofilatos, K.; Treille, D.; Urscheler, C.; Wallny, R.; Weber, H. A.; Wehrli, L.] Swiss Fed Inst Technol, Inst Particle Phys, Zurich, Switzerland. [Aguilo, E.; Amsler, C.; Chiochia, V.; De Visscher, S.; Favaro, C.; Rikova, M. Ivova; Mejias, B. Millan; Otiougova, P.; Robmann, P.; Snoek, H.; Tupputi, S.; Verzetti, M.] Univ Zurich, Zurich, Switzerland. [Chang, Y. H.; Chen, K. H.; Kuo, C. M.; Li, S. W.; Lin, W.; Liu, Z. K.; Lu, Y. J.; Mekterovic, D.; Singh, A. P.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Dietz, C.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wan, X.; Wang, M.] Natl Taiwan Univ NTU, Taipei, Taiwan. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Karapinar, G.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, L. N.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Yildirim, E.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey. [Cankocak, K.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. Univ Bucharest, Fac Phys, Bucharest, Romania. [Belyaev, A.; Worm, S. D.; Basso, L.; Bell, K. W.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Jackson, J.; Kennedy, B. W.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Womersley, W. J.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Bakirci, M. N.; Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey. [Cerci, S.; Cerci, D. Sunar; Tali, B.] Adiyaman Univ, Adiyaman, Turkey. [Ozturk, S.] Univ Iowa, Iowa City, IA USA. [Sogut, K.] Mersin Univ, Mersin, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Kaya, M.; Kaya, O.] Kafkas Univ, Kars, Turkey. [Ozkorucuklu, S.] Suleyman Demirel Univ, TR-32200 Isparta, Turkey. [Sonmez, N.] Ege Univ, Izmir, Turkey. [Hatakeyama, K.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Liu, H.; Babb, J.; Clare, R.; Dinardo, M. E.; Gary, J. W.; Giordano, F.; Hanson, G.; Jeng, G. Y.; Long, O. R.; Luthra, A.; Nguyen, H.; Paramesvaran, S.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sharma, V.; Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; Evans, D.; Golf, F.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Macneill, I.; Mangano, B.; Padhi, S.; Palmer, C.; Petrucciani, G.; Pieri, M.; Sani, M.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bellan, R.; Campagnari, C.; D'Alfonso, M.; Danielson, T.; Flowers, K.; Geffert, P.; Incandela, J.; Justus, C.; Kalavase, P.; Koay, S. A.; Kovalskyi, D.; Krutelyov, V.; Lowette, S.; Mccoll, N.; Pavlunin, V.; Rebassoo, F.; Ribnik, J.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Akgun, B.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Liu, Y. F.; Paulini, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Edelmaier, C. J.; Ford, W. T.; Gaz, A.; Heyburn, B.; Lopez, E. Luiggi; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Eggert, N.; Gibbons, L. K.; Heltsley, B.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Vaughan, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Bauerdick, L. A. 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I.; Dahmes, B.; De Benedetti, A.; Franzoni, G.; Gude, A.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Sasseville, M.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Cremaldi, L. M.; Kroeger, R.; Perera, L.; Rahmat, R.; Sanders, D. A.] Univ Mississippi, University, MS 38677 USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Butt, J.; Claes, D. R.; Dominguez, A.; Eads, M.; Keller, J.; Kravchenko, I.; Lazo-Flores, J.; Malbouisson, H.; Malik, S.; Snow, G. R.] Univ Nebraska Lincoln, Lincoln, NE USA. [Baur, U.; Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Kumar, A.; Shipkowski, S. P.; Smith, K.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Nash, D.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Anastassov, A.; Kubik, A.; Mucia, N.; Odell, N.; Ofierzynski, R. 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W.; Balazs, M.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Lin, C.; Neu, C.; Wood, J.; Yohay, R.] Univ Virginia, Charlottesville, VA USA. [Gollapinni, S.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sakharov, A.] Wayne State Univ, Detroit, MI USA. [Anderson, M.; Bachtis, M.; Belknap, D.; Borrello, L.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Friis, E.; Gray, L.; Grogg, K. S.; Grothe, M.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Klukas, J.; Lanaro, A.; Lazaridis, C.; Leonard, J.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Palmonari, F.; Pierro, G. A.; Ross, I.; Savin, A.; Smith, W. H.; Swanson, J.] Univ Wisconsin, Madison, WI 53706 USA. RP Chatrchyan, S (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Gerbaudo, Davide/J-4536-2012; Andreev, Vladimir/M-8665-2015; TUVE', Cristina/P-3933-2015; KIM, Tae Jeong/P-7848-2015; Arce, Pedro/L-1268-2014; Flix, Josep/G-5414-2012; Azarkin, Maxim/N-2578-2015; Paganoni, Marco/A-4235-2016; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Seixas, Joao/F-5441-2013; Sznajder, Andre/L-1621-2016; Vilela Pereira, Antonio/L-4142-2016; Xie, Si/O-6830-2016; Sen, Sercan/C-6473-2014; D'Alessandro, Raffaello/F-5897-2015; Belyaev, Alexander/F-6637-2015; Stahl, Achim/E-8846-2011; Trocsanyi, Zoltan/A-5598-2009; Konecki, Marcin/G-4164-2015; Bedoya, Cristina/K-8066-2014; My, Salvatore/I-5160-2015; Matorras, Francisco/I-4983-2015; Ragazzi, Stefano/D-2463-2009; Dremin, Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Leonidov, Andrey/M-4440-2013; de la Cruz, Begona/K-7552-2014; Scodellaro, Luca/K-9091-2014; Josa, Isabel/K-5184-2014; Calvo Alamillo, Enrique/L-1203-2014; Paulini, Manfred/N-7794-2014; Vogel, Helmut/N-8882-2014; Marinho, Franciole/N-8101-2014; Ferguson, Thomas/O-3444-2014; Benussi, Luigi/O-9684-2014; Grandi, Claudio/B-5654-2015; Leonidov, Andrey/P-3197-2014; Bernardes, Cesar Augusto/D-2408-2015; Lazzizzera, Ignazio/E-9678-2015; Markina, Anastasia/E-3390-2012; Dogangun, Oktay/L-9252-2013; Marlow, Daniel/C-9132-2014; Oguri, Vitor/B-5403-2013; Janssen, Xavier/E-1915-2013; Bartalini, Paolo/E-2512-2014; Codispoti, Giuseppe/F-6574-2014; Gribushin, Andrei/J-4225-2012; Cerrada, Marcos/J-6934-2014; Azzi, Patrizia/H-5404-2012; Calderon, Alicia/K-3658-2014; Fruhwirth, Rudolf/H-2529-2012; de Jesus Damiao, Dilson/G-6218-2012; Rolandi, Luigi (Gigi)/E-8563-2013; Montanari, Alessandro/J-2420-2012; Raidal, Martti/F-4436-2012; Tomei, Thiago/E-7091-2012; Zalewski, Piotr/H-7335-2013; Ivanov, Andrew/A-7982-2013; Hill, Christopher/B-5371-2012; Liu, Sheng/K-2815-2013; Zhukov, Valery/K-3615-2013; Venturi, Andrea/J-1877-2012; Wimpenny, Stephen/K-8848-2013; Kadastik, Mario/B-7559-2008; Mundim, Luiz/A-1291-2012; De La Cruz Burelo, Eduard/B-9802-2013; Bagliesi, Giuseppe/C-2230-2013; Petrushanko, Sergey/D-6880-2012; Santaolalla, Javier/C-3094-2013; Alves, Gilvan/C-4007-2013; Tinoco Mendes, Andre David/D-4314-2011; Novaes, Sergio/D-3532-2012; Wulz, Claudia-Elisabeth/H-5657-2011; tosi, mia/J-5777-2012; Della Ricca, Giuseppe/B-6826-2013 OI Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Gerbaudo, Davide/0000-0002-4463-0878; TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; Arce, Pedro/0000-0003-3009-0484; Flix, Josep/0000-0003-2688-8047; Paganoni, Marco/0000-0003-2461-275X; Gulmez, Erhan/0000-0002-6353-518X; Seixas, Joao/0000-0002-7531-0842; Sznajder, Andre/0000-0001-6998-1108; Vilela Pereira, Antonio/0000-0003-3177-4626; Xie, Si/0000-0003-2509-5731; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Belyaev, Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279; Konecki, Marcin/0000-0001-9482-4841; Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680; Matorras, Francisco/0000-0003-4295-5668; Ragazzi, Stefano/0000-0001-8219-2074; Scodellaro, Luca/0000-0002-4974-8330; Calvo Alamillo, Enrique/0000-0002-1100-2963; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Marinho, Franciole/0000-0002-7327-0349; Ferguson, Thomas/0000-0001-5822-3731; Benussi, Luigi/0000-0002-2363-8889; Grandi, Claudio/0000-0001-5998-3070; Lazzizzera, Ignazio/0000-0001-5092-7531; Dogangun, Oktay/0000-0002-1255-2211; Codispoti, Giuseppe/0000-0003-0217-7021; Cerrada, Marcos/0000-0003-0112-1691; Azzi, Patrizia/0000-0002-3129-828X; de Jesus Damiao, Dilson/0000-0002-3769-1680; Rolandi, Luigi (Gigi)/0000-0002-0635-274X; Montanari, Alessandro/0000-0003-2748-6373; Tomei, Thiago/0000-0002-1809-5226; Ivanov, Andrew/0000-0002-9270-5643; Hill, Christopher/0000-0003-0059-0779; Wimpenny, Stephen/0000-0003-0505-4908; Mundim, Luiz/0000-0001-9964-7805; De La Cruz Burelo, Eduard/0000-0002-7469-6974; Tinoco Mendes, Andre David/0000-0001-5854-7699; Novaes, Sergio/0000-0003-0471-8549; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Della Ricca, Giuseppe/0000-0003-2831-6982 FU BMWF (Austria); FWF (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MES (Bulgaria); CERN; CAS (China); MoST (China); NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); MoER (Estonia) [SF0690030s09]; ERDF (Estonia); Academy of Finland (Finland); MEC (Finland); HIP (Finland); CEA (France); CNRS/IN2P3 (France); BMBF (Germany); DFG (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NKTH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF (Korea); WCU (Korea); LAS (Lithuania); CINVESTAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); MSI (New Zealand); PAEC (Pakistan); MSHE (Poland); NSC (Poland); FCT (Portugal); JINR (Armenia); JINR (Belarus); JINR (Georgia); JINR (Ukraine); JINR (Uzbekistan); MON (Russia); RosAtom (Russia); RAS (Russia); RFBR (Russia); MSTD (Serbia); SEIDI (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); ThEP (Thailand); IPST (Thailand); NECTEC (Thailand); TUBITAK (Turkey); TAEK (Turkey); NASU (Ukraine); STFC (United Kingdom); DOE (USA); NSF (USA); Marie-Curie programme (European Union); European Research Council (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Austrian Science Fund (FWF); Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of Czech Republic; Council of Science and Industrial Research, India; Compagnia di San Paolo (Torino); HOMING PLUS programme of Foundation for Polish Science; European Union, Regional Development Fund FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC machine. We thank the technical and administrative staff at CERN and other CMS institutes, and acknowledge support from BMWF and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); MoER, SF0690030s09 and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NKTH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF and WCU (Korea); LAS (Lithuania); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MSI (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Armenia, Belarus, Georgia, Ukraine, Uzbekistan); MON, RosAtom, RAS and RFBR (Russia); MSTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); ThEP, IPST and NECTEC (Thailand); TUBITAK and TAEK (Turkey); NASU (Ukraine); STFC (United Kingdom); DOE and NSF (USA).; Individuals have received support from the Marie-Curie programme and the European Research Council (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Austrian Science Fund (FWF); the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of Czech Republic; the Council of Science and Industrial Research, India; the Compagnia di San Paolo (Torino); and the HOMING PLUS programme of Foundation for Polish Science, cofinanced from European Union, Regional Development Fund. NR 50 TC 11 Z9 11 U1 0 U2 61 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. 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CA CMS Collaboration TI Search for the standard model Higgs boson produced in association with W and Z bosons in pp collisions at root s=7 TeV SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering ID PARTON DISTRIBUTIONS; MASSLESS PARTICLES; BROKEN SYMMETRIES; LHC; MASSES AB A search for the Higgs boson produced in association with a W or Z boson in proton-proton collisions at a center-of-mass energy of 7 TeV is performed with the CMS detector at the LHC using the full 2011 data sample, from an integrated luminosity of 5 fb(-1). Higgs boson decay modes to tau tau and WW are explored by selecting events with three or four leptons in the final state. No excess above background expectations is observed, resulting in exclusion limits on the product of Higgs associated production cross section and decay branching fraction for Higgs boson masses between 110 and 200 GeV in these channels. Combining these results with other CMS associated production searches using the same dataset in the H -> gamma gamma and H -> b (b) over bar decay modes, the cross section for associated Higgs boson production 3.3 times the standard model expectation or larger is ruled out at the 95% confidence level for a Higgs boson mass of 125 GeV. C1 [Chatrchyan, S.; Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.; CMS Collaboration] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Aguilo, E.; Bergauer, T.; Dragicevic, M.; Ero, J.; Fabjan, C.; Friedl, M.; Fruehwirth, R.; Ghete, V. M.; Hammer, J.; Hormann, N.; Hrubec, J.; Jeitler, M.; Kiesenhofer, W.; Knunz, V.; Krammer, M.; Liko, D.; Mikulec, I.; Pernicka, M.; Rahbaran, B.; Rohringer, C.; Rohringer, H.; Schofbeck, R.; Strauss, J.; Taurok, A.; Waltenberger, W.; Walzel, G.; Widl, E.; Wulz, C. -E.] Inst Hochenergiephys OeAW, Vienna, Austria. [Mossolov, V.; Shumeiko, N.; Gonzalez, J. Suarez] Natl Ctr Particle & High Energy Phys, Minsk, Byelarus. 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[Kumar, Ashok; Kumar, Arun; Ahuja, S.; Bhardwaj, A.; Choudhary, B. C.; Malhotra, S.; Naimuddin, M.; Ranjan, K.; Sharma, V.; Shivpuri, R. K.] Univ Delhi, Delhi 110007, India. [Banerjee, S.; Bhattacharya, S.; Dutta, S.; Gomber, B.; Jain, Sa.; Jain, Sh.; Khurana, R.; Sarkar, S.; Sharan, M.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Choudhury, R. K.; Dutta, D.; Kailas, S.; Kumar, V.; Mehta, P.; Mohanty, A. K.; Pant, L. M.; Shukla, P.] Bhabha Atom Res Ctr, Mumbai 400085, Maharashtra, India. [Aziz, T.; Ganguly, S.; Guchait, M.; Maity, M.; Majumder, G.; Mazumdar, K.; Mohanty, G. B.; Parida, B.; Sudhakar, K.; Wickramage, N.] Tata Inst Fundamental Res EHEP, Bombay, Maharashtra, India. [Banerjee, S.; Dugad, S.] Tata Inst Fundamental Res HECR, Bombay, Maharashtra, India. [Arfaei, H.; Bakhshiansohi, H.; Etesami, S. M.; Fahim, A.; Hashemi, M.; Hesari, H.; Jafari, A.; Khakzad, M.; Najafabadi, M. Mohammadi; Mehdiabadi, S. 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M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Meneghelli, M.; Montanari, A.; Navarria, F. L.; Odorici, F.; Perrotta, A.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Travaglini, R.] INFN Sez Bologna, Bologna, Italy. [Bonacorsi, D.; Brigliadori, L.; Capiluppi, P.; Castro, A.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Meneghelli, M.; Navarria, F. L.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] INFN Sez Catania, Catania, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. INFN Sez Firenze, Florence, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gallo, E.; Gonzi, S.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] Univ Florence, Florence, Italy. [Fabbri, F.; Benussi, L.; Bianco, S.; Colafranceschi, S.; Piccolo, D.] INFN Lab Nazl Frascati, Frascati, Italy. INFN Sez Genova, Genoa, Italy. [Fabbricatore, P.; Musenich, R.; Tosi, S.] Univ Genoa, Genoa, Italy. INFN Sez Milano Bicocca, Milan, Italy. [Benaglia, A.; De Guio, F.; Di Matteo, L.; Fiorendi, S.; Gennai, S.; Ghezzi, A.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Massironi, A.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; Sala, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Montoya, C. A. Carrillo; Cavallo, N.; De Cosa, A.; Dogangun, O.; Fabozzi, F.; Iorio, A. O. M.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.] INFN Sez Napoli, Naples, Italy. [Azzi, P.; Bacchetta, N.; Bisello, D.; Branca, A.; Carlin, R.; Checchia, P.; Dorigo, T.; Gasparini, F.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Lazzizzera, I.; Margoni, M.; Meneguzzo, A. T.; Montecassiano, F.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Vanini, S.; Zotto, P.; Zucchetta, A.; Zumerle, G.] INFN Sez Padova, Padua, Italy. [Bisello, D.; Branca, A.; Carlin, R.; Gasparini, F.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Vanini, S.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.; Lazzizzera, I.] Univ Trent, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Torre, P.; Vitulo, P.] INFN Sez Pavia, Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Torre, P.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Fano, L.; Lariccia, P.; Lucaroni, A.; Mantovani, G.; Menichelli, M.; Nappi, A.; Romeo, F.; Saha, A.; Santocchia, A.; Spiezia, A.; Taroni, S.] INFN Sez Perugia, Perugia, Italy. [Biasini, M.; Bilei, G. M.; Fano, L.; Lariccia, P.; Lucaroni, A.; Mantovani, G.; Nappi, A.; Romeo, F.; Santocchia, A.; Spiezia, A.; Taroni, S.] Univ Perugia, I-06100 Perugia, Italy. [Azzurri, P.; Bagliesi, G.; Boccali, T.; Broccolo, G.; Castaldi, R.; Dell'Orso, R.; Fiori, F.; Foa, L.; Giassi, A.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] INFN Sez Pisa, Pisa, Italy. [Fiori, F.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Azzurri, P.; Broccolo, G.; D'Agnolo, R. T.; Foa, L.; Ligabue, F.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Diemoz, M.; Grassi, M.; Longo, E.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Sigamani, M.; Soffi, L.; Rovelli, C.] INFN Sez Roma, Rome, Italy. [Barone, L.; Del Re, D.; Grassi, M.; Longo, E.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Soffi, L.; Rovelli, C.] Univ Roma La Sapienza, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Biino, C.; Cartiglia, N.; Costa, M.; Demaria, N.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Pastrone, N.; Pelliccioni, M.; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Pereira, A. Vilela] INFN Sez Torino, Turin, Italy. [Amapane, N.; Argiro, S.; Costa, M.; Migliore, E.; Monaco, V.; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; Marone, M.; Montanino, D.; Penzo, A.; Schizzi, A.] INFN Sez Trieste, Trieste, Italy. [Della Ricca, G.; Montanino, D.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Heo, S. G.; Kim, T. Y.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Chang, S.; Kim, D. H.; Kim, G. N.; Kong, D. J.; Park, H.; Ro, S. R.; Son, D. C.; Son, T.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, J. Y.; Kim, Zero J.; Song, S.] Chonnam Natl Univ, Inst Univ & Elementary Particles, Kwangju, South Korea. [Choi, S.; Cyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, T. J.; Lee, K. S.; Moon, D. H.; Park, S. K.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Cho, Y.; Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. S.; Kwon, E.; Lee, B.; Lee, J.; Lee, S.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Bilinskas, M. J.; Grigelionis, I.; Janulis, M.; Juodagalvis, A.] Vilnius State Univ, Vilnius, Lithuania. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Lopez-Fernandez, R.; Magana Villalba, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] Ctr Invest & Estudios Avanzados IPN, Mexico City, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.; Reyes-Santos, M. A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Bell, A. J.; Butler, P. H.; Doesburg, R.; Reucroft, S.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Asghar, M. I.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Boimska, B.; Frueboes, T.; Gokieli, R.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.] Univ Warsaw, Fac Phys, Inst Expt Phys, Warsaw, Poland. [Almeida, N.; Bargassa, P.; David, A.; Faccioli, P.; Parracho, P. G. Ferreira; Gallinaro, M.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao Fis Expt Particulas, Lisbon, Portugal. [Tsamalaidze, Z.; Bunin, P.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Kozlov, G.; Lanev, A.; Malakhov, A.; Moisenz, P.; Palichik, V.; Perelygin, V.; Savina, M.; Shmatov, S.; Smirnov, V.; Volodko, A.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Evstyukhin, S.; Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, Gatchina, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Matveev, V.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Russian Acad Sci, Inst Nucl Res, Moscow, Russia. [Epshteyn, V.; Erofeeva, M.; Gavrilov, V.; Kossov, M.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Stolin, V.; Vlasov, E.; Zhokin, A.; Starodumov, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Zhukov, V.; Katkov, I.; Belyaev, A.; Boos, E.; Bunichev, V.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Markina, A.; Obraztsov, S.; Lov, M. Per Fi; Petrushanko, S.; Popov, A.; Sarycheva, L.; Savrin, V.] Moscow MV Lomonosov State Univ, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Grishin, V.; Kachanov, V.; Konstantinov, D.; Korablev, A.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Serban, A. T.; Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Alcaraz Maestre, J.; Arce, P.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.; Willmott, C.] Ctr Invest Energet Medioambient & Tecnol CIEMAT, Madrid, Spain. [Albajar, C.; Codispoti, G.; de Troconiz, J. F.] Univ Autonoma Madrid, Madrid, Spain. [Bruno, G.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.; Piedra Gomez, J.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Chuang, S. H.; Duarte Campderros, J.; Felcini, M.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Graziano, A.; Jorda, C.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Sobron Sanudo, M.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Genchev, V.; Iaydjiev, P.; Puljak, I.; Chierici, R.; Guthoff, M.; Hauth, T.; Foudas, C.; Hajdu, C.; Mohanty, A. K.; Calabria, C.; De Filippis, N.; Tropiano, A.; Benaglia, A.; Di Matteo, L.; Gennai, S.; Montoya, C. A. Carrillo; De Cosa, A.; Paolucci, P.; Bacchetta, N.; Branca, A.; Tosi, M.; Lucaroni, A.; Taroni, S.; Squillacioti, P.; Tonelli, G.; Venturi, A.; Del Re, D.; Grassi, M.; Meridiani, P.; Mariotti, C.; Musich, M.; Marone, M.; Montanino, D.; Kossov, M.; Grishin, V.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Baillon, P.; Ball, A. H.; Barney, D.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Perez, J. A. Coarasa; D'Enterria, D.; Dabrowski, A.; De Roeck, A.; Di Guida, S.; Dobson, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Frisch, B.; Funk, W.; Georgiou, G.; Giffels, M.; Gigi, D.; Gill, K.; Giordano, D.; Giunta, M.; Glege, F.; Garrido, R. Gomez-Reino; Govoni, P.; Gowdy, S.; Guida, R.; Hansen, M.; Harris, P.; Hartl, C.; Harvey, J.; Hegner, B.; Hinzmann, A.; Innocente, V.; Janot, P.; Kaadze, K.; Karavakis, E.; Kousouris, K.; Lecoq, P.; Lee, Y. -J.; Lenzi, P.; Lourenco, C.; Maeki, T.; Malberti, M.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moser, R.; Mozer, M. U.; Mulders, M.; Musella, P.; Nesvold, E.; Orimoto, T.; Orsini, L.; Cortezon, E. Palencia; Perez, E.; Perrozzi, L.; Petrilli, A.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Piparo, D.; Polese, G.; Quertenmont, L.; Racz, A.; Reece, W.; Antunes, J. Rodrigues; Rolandi, G.; Rommerskirchen, T.; Rovelli, C.; Rovere, M.; Sakulin, H.; Santanastasio, F.; Schaefer, C.; Schwick, C.; Segoni, I.; Sekmen, S.; Sharma, A.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Tsirou, A.; Veres, G. I.; Vlimant, J. R.; Woehri, H. K.; Worm, S. D.; Zeuner, W. D.; Pela, J.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Gabathuler, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Meier, F.; Renker, D.; Rohe, T.; Sibille, J.; Naegeli, C.] Paul Scherrer Inst, Villigen, Switzerland. [Baeni, L.; Bortignon, P.; Buchmann, M. A.; Casal, B.; Chanon, N.; Deisher, A.; Dissertori, G.; Dittmar, M.; Duenser, M.; Eugster, J.; Freudenreich, K.; Grab, C.; Hits, D.; Lecomte, P.; Lustermann, W.; Marini, A. C.; del Arbol, P. Martinez Ruiz; Mohr, N.; Moortgat, F.; Naegeli, C.; Nef, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pape, L.; Pauss, F.; Peruzzi, M.; Ronga, F. J.; Rossini, M.; Sala, L.; Sanchez, A. K.; Starodumov, A.; Stieger, B.; Takahashi, M.; Tauscher, L.; Thea, A.; Theofilatos, K.; Treille, D.; Urscheler, C.; Wallny, R.; Weber, H. A.; Wehrli, L.] ETH, Inst Particle Phys, Zurich, Switzerland. [Amsler, C.; Chiochia, V.; De Visscher, S.; Favaro, C.; Rikova, M. Ivova; Mejias, B. Millan; Otiougova, P.; Robmann, P.; Snoek, H.; Tupputi, S.; Verzetti, M.] Univ Zurich, Zurich, Switzerland. [Chang, Y. H.; Chen, K. H.; Kuo, C. M.; Li, S. W.; Lin, W.; Liu, Z. K.; Lu, Y. J.; Mekterovic, D.; Singh, A. P.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Dietz, C.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wan, X.; Wang, M.] Natl Taiwan Univ NTU, Taipei, Taiwan. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Karaman, T.; Karapinar, G.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, L. N.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Yildirim, E.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey. [Cankocak, K.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Bostock, F.; Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Kreczko, L.; Metson, S.; Newbold, D. M.; Nirunpong, K.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Worm, S. D.; Basso, L.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Jackson, J.; Kennedy, B. W.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Womersley, W. J.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Bainbridge, R.; Ball, G.; Beuselinck, R.; Buchmuller, O.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Papageorgiou, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Ryan, M. J.; Seez, C.; Sharp, P.; Sparrow, A.; Stoye, M.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.; Whyntie, T.] Univ London Imperial Coll Sci Technol & Med, London, England. [Abdulsalam, A.; Chadwick, M.; Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Hatakeyama, K.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; John, J. St.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Bhattacharya, S.; Cutts, D.; Ferapontov, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Nguyen, D.; Segala, M.; Sinthuprasith, T.; Speer, T.; Tsang, K. V.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Dolen, J.; Erbacher, R.; Gardner, M.; Houtz, R.; Ko, W.; Kopecky, A.; Lander, R.; Miceli, T.; Pellett, D.; Ricci-tam, F.; Rutherford, B.; Searle, M.; Smith, J.; Squires, M.; Tripathi, M.; Sierra, R. Vasquez] Univ Calif Davis, Davis, CA 95616 USA. [Andreev, V.; Cline, D.; Cousins, R.; Duris, J.; Erhan, S.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Plager, C.; Rakness, G.; Schlein, P.; Tucker, J.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Babb, J.; Clare, R.; Dinardo, M. E.; Ellison, J.; Gary, J. W.; Giordano, F.; Hanson, G.; Jeng, G. Y.; Liu, H.; Long, O. R.; Luthra, A.; Nguyen, H.; Paramesvaran, S.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; Evans, D.; Golf, F.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Macneill, I.; Mangano, B.; Padhi, S.; Palmer, C.; Petrucciani, G.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bellan, R.; Campagnari, C.; D'Alfonso, M.; Danielson, T.; Flowers, K.; Geffert, P.; Incandela, J.; Justus, C.; Kalavase, P.; Koay, S. A.; Kovalskyi, D.; Krutelyov, V.; Lowette, S.; Mccoll, N.; Pavlunin, V.; Rebassoo, F.; Ribnik, J.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dias, F. A.; Apresyan, A.; Bornheim, A.; Chen, Y.; DiMarco, E.; Duarte, J.; Gataullin, M.; Ma, Y.; Mott, A.; Newman, H. B.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Traczyk, P.; Veverka, J.; Wilkinson, R.; Yang, Y.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Akgun, B.; Azzolini, V.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Liu, Y. F.; Paulini, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Edelmaier, C. J.; Ford, W. T.; Gaz, A.; Heyburn, B.; Lopez, E. Luiggi; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Eggert, N.; Gibbons, L. K.; Heltsley, B.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Vaughan, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bloch, I.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Green, D.; Gutsche, O.; Hanlon, J.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Kilminster, B.; Klima, B.; Kunori, S.; Kwan, S.; Leonidopoulos, C.; Linacre, J.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Tan, P.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Wu, W.; Yang, F.; Yumiceva, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Chen, M.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Drozdetskiy, A.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Gartner, J.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Remington, R.; Rinkevicius, A.; Sellers, P.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Hewamanage, S.; Lebolo, L. M.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Gleyzer, S. V.; Haas, J.; Hagopian, S.; Hagopian, V.; Jenkins, M.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Vodopiyanov, I.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Anghel, I. M.; Apanasevich, L.; Bai, Y.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Callner, J.; Cavanaugh, R.; Dragoiu, C.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Lacroix, F.; Malek, M.; O'Brien, C.; Silkworth, C.; Strom, D.; Varelas, N.] Univ Illinois Chicago UIC, Chicago, IL USA. [Ozturk, S.; Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Duru, F.; Griffiths, S.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Newsom, C. R.; Norbeck, E.; Onel, Y.; Ozok, F.; Sen, S.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Giurgiu, G.; Gritsan, A. V.; Guo, Z. J.; Hu, G.; Maksimovic, P.; Rappoccio, S.; Swartz, M.; Whitbeck, A.] Johns Hopkins Univ, Baltimore, MD USA. [Sibille, J.; Baringer, P.; Bean, A.; Benelli, G.; Grachov, O.; Kenny, R. P., III; Murray, M.; Noonan, D.; Sanders, S.; Stringer, R.; Tinti, G.; Wood, J. S.; Zhukova, V.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Bolton, T.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Boutemeur, M.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kirn, M.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Peterman, A.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.; Twedt, E.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Bauer, G.; Bendavid, J.; Busza, W.; Butz, E.; Cali, I. A.; Chan, M.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Hahn, K. A.; Kim, Y.; Klute, M.; Krajczar, K.; Li, W.; Luckey, P. D.; Ma, T.; Nahn, S.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Rudolph, M.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Sung, K.; Velicanu, D.; Wenger, E. A.; Wolf, R.; Wyslouch, B.; Xie, S.; Yang, M.; Yilmaz, Y.; Yoon, A. S.; Zanetti, M.] MIT, Cambridge, MA 02139 USA. [Cooper, S. I.; Dahmes, B.; De Benedetti, A.; Franzoni, G.; Gude, A.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Sasseville, M.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Cremaldi, L. M.; Kroeger, R.; Perera, L.; Rahmat, R.; Sanders, D. A.] Univ Mississippi, University, MS 38677 USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Butt, J.; Claes, D. R.; Dominguez, A.; Eads, M.; Keller, J.; Kravchenko, I.; Lazo-Flores, J.; Malbouisson, H.; Malik, S.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Baur, U.; Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Kumar, A.; Shipkowski, S. P.; Smith, K.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Nash, D.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Anastassov, A.; Kubik, A.; Mucia, N.; Odell, N.; Ofierzynski, R. A.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Antonelli, L.; Berry, D.; Brinkerhoff, A.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kolb, J.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Morse, D. M.; Pearson, T.; Ruchti, R.; Slaunwhite, J.; Valls, N.; Wayne, M.; Wolf, M.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Abdulsalam, A.; Bylsma, B.; Durkin, L. S.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Puigh, D.; Rodenburg, M.; Vuosalo, C.; Williams, G.; Winer, B. L.] Ohio State Univ, Columbus, OH 43210 USA. [Adam, N.; Berry, E.; Elmer, P.; Gerbaudo, D.; Halyo, V.; Hebda, P.; Hegeman, J.; Hunt, A.; Jindal, P.; Pegna, D. Lopes; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Raval, A.; Safdi, B.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Safdi, B.; Acosta, J. G.; Brownson, E.; Huang, X. T.; Lopez, A.; Mendez, H.; Oliveros, S.; Vargas, J. E. Ramirez; Zatserklyaniy, A.] Univ Puerto Rico, Mayaguez, PR USA. [Abdulsalam, A.; Adiguzel, A.; Safdi, B.; Alagoz, E.; Barnes, V. E.; Benedetti, D.; Bolla, G.; Bortoletto, D.; De Mattia, M.; Everett, A.; Hu, Z.; Jones, M.; Koybasi, O.; Kress, M.; Laasanen, A. T.; Leonardo, N.; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Marono, M. Vidal; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Guragain, S.; Parashar, N.] Purdue Univ Calumet, Hammond, LA USA. [Safdi, B.; Adair, A.; Boulahouache, C.; Ecklund, K. M.; Geurts, F. J. M.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Safdi, B.; Betchart, B.; Bodek, A.; Chung, Y. S.; Covarelli, R.; De Barbaro, P.; Demina, R.; Eshaq, Y.; Garcia-Bellido, A.; Goldenzweig, P.; Harel, J. Han A.; Miner, D. C.; Vishnevskiy, D.; Zielinski, M.] Univ Rochester, Rochester, NY 14627 USA. [Safdi, B.; Bhatti, A.; Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Malik, S.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA. [Safdi, B.; Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Lath, A.; Panwalkar, S.; Park, M.; Patel, R.; Rekovic, V.; Robles, J.; Rose, K.; Salur, S.; Schnetzer, S.; Seitz, C.; Somalwar, S.; Stone, R.; Thomas, S.] Rutgers State Univ, Piscataway, NJ USA. [Cerizza, G.; Hollingsworth, M.; Spanier, S.; Yang, Z. C.; York, A.] Univ Tennessee, Knoxville, TN USA. [Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Khotilovich, V.; Montalvo, R.; Osipenkov, I.; Pakhotin, Y.; Perloff, A.; Roe, J.; Safonov, A.; Sakuma, T.; Sengupta, S.; Suarez, I.; Tatarinov, A.; Toback, D.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Damgov, J.; Dudero, P. R.; Jeong, C.; Kovitanggoon, K.; Lee, S. W.; Libeiro, T.; Roh, Y.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Appelt, E.; Delannoy, A. G.; Florez, C.; Greene, S.; Gurrola, A.; Johns, W.; Johnston, C.; Kurt, P.; Maguire, C.; Melo, A.; Sharma, M.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN USA. [Arenton, M. W.; Balazs, M.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Lin, C.; Neu, C.; Wood, J.; Yohay, R.] Univ Virginia, Charlottesville, VA USA. [Gollapinni, S.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sakharov, A.] Wayne State Univ, Detroit, MI USA. [Anderson, M.; Bachtis, M.; Belknap, D.; Borrello, L.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Friis, E.; Gray, L.; Grogg, K. S.; Grothe, M.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Klukas, J.; Lanaro, A.; Lazaridis, C.; Leonard, J.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Palmonari, F.; Pierro, G. A.; Ross, I.; Savin, A.; Smith, W. H.; Swanson, J.] Univ Wisconsin, Madison, WI 53706 USA. [Fabjan, C.; Fruehwirth, R.; Krammer, M.; Wulz, C. -E.] Vienna Univ Technol, A-1040 Vienna, Austria. [Giammanco, A.] NICPB, Tallinn, Estonia. [Bernardes, C. A.; Gregores, E. M.; Mercadante, P. G.] Univ Fed ABC, Santo Andre, Brazil. [Assran, Y.] Suez Canal Univ, Suez, Egypt. [Elgammal, S.; Khalil, S.] Zewail City Sci & Technol, Zewail, Egypt. [Kamel, A. Ellithi] Cairo Univ, Cairo, Egypt. [Mahmoud, M. A.] Fayoum Univ, Al Fayyum, Egypt. [Radi, A.] British Univ, Cairo, Egypt. [Radi, A.] Ain Shams Univ, Cairo, Egypt. [Bluj, M.] Natl Ctr Nucl Res, Otwock, Poland. [Agram, J. -L.; Conte, E.; Drouhin, F.; Fontaine, J. -C.] Univ Haute Alsace, Mulhouse, France. [Bergholz, M.; Lohmann, W.; Schmidt, R.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Horvath, D.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Vesztergombi, G.] Eotvos Lorand Univ, Budapest, Hungary. [Guchait, M.] Tata Inst Fundamental Res HECR, Mumbai, Maharashtra, India. [Maity, M.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Bakhshiansohi, H.; Fahim, A.; Jafari, A.] Sharif Univ Technol, Tehran, Iran. [Etesami, S. M.; Zeinali, M.] Isfahan Univ Technol, Esfahan, Iran. [Safarzadeh, B.] Islamic Azad Univ, Plasma Phys Res Ctr, Sci & Res Branch, Tehran, Iran. [Colafranceschi, S.] Univ Rome, Fac Ingn, Rome, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata, I-85100 Potenza, Italy. [Meola, S.] Univ Guglielmo Marconi, Rome, Italy. [Martini, L.] Univ Siena, I-53100 Siena, Italy. [Serban, A. T.] Univ Bucharest, Fac Phys, Bucharest, Romania. [Rolandi, G.] Scuola Normale Sez INFN, Pisa, Italy. [Sphicas, P.] Univ Athens, Athens, Greece. [Bakirci, M. N.; Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey. [Cerci, S.; Cerci, D. Sunar; Tali, B.] Adiyaman Univ, Adiyaman, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Sogut, K.] Mersin Univ, Mersin, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Kaya, M.; Kaya, O.] Kafkas Univ, Kars, Turkey. 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RI Calderon, Alicia/K-3658-2014; de la Cruz, Begona/K-7552-2014; Scodellaro, Luca/K-9091-2014; Josa, Isabel/K-5184-2014; Calvo Alamillo, Enrique/L-1203-2014; Paulini, Manfred/N-7794-2014; Vogel, Helmut/N-8882-2014; Marinho, Franciole/N-8101-2014; Ferguson, Thomas/O-3444-2014; Benussi, Luigi/O-9684-2014; Dahms, Torsten/A-8453-2015; Grandi, Claudio/B-5654-2015; Markina, Anastasia/E-3390-2012; Dogangun, Oktay/L-9252-2013; Marlow, Daniel/C-9132-2014; de Jesus Damiao, Dilson/G-6218-2012; Oguri, Vitor/B-5403-2013; Janssen, Xavier/E-1915-2013; Bartalini, Paolo/E-2512-2014; Codispoti, Giuseppe/F-6574-2014; Gribushin, Andrei/J-4225-2012; Cerrada, Marcos/J-6934-2014; Azzi, Patrizia/H-5404-2012; Fruhwirth, Rudolf/H-2529-2012; Rolandi, Luigi (Gigi)/E-8563-2013; Montanari, Alessandro/J-2420-2012; Raidal, Martti/F-4436-2012; Tomei, Thiago/E-7091-2012; Zalewski, Piotr/H-7335-2013; Ivanov, Andrew/A-7982-2013; Hill, Christopher/B-5371-2012; Liu, Sheng/K-2815-2013; Zhukov, Valery/K-3615-2013; Venturi, Andrea/J-1877-2012; Wimpenny, Stephen/K-8848-2013; Mundim, Luiz/A-1291-2012; De La Cruz Burelo, Eduard/B-9802-2013; Petrushanko, Sergey/D-6880-2012; Santaolalla, Javier/C-3094-2013; Alves, Gilvan/C-4007-2013; Tinoco Mendes, Andre David/D-4314-2011; Novaes, Sergio/D-3532-2012; Wulz, Claudia-Elisabeth/H-5657-2011; tosi, mia/J-5777-2012; Lokhtin, Igor/D-7004-2012; Della Ricca, Giuseppe/B-6826-2013; Kadastik, Mario/B-7559-2008; Seixas, Joao/F-5441-2013; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Gerbaudo, Davide/J-4536-2012; Dremin, Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Leonidov, Andrey/M-4440-2013; Andreev, Vladimir/M-8665-2015; Matorras, Francisco/I-4983-2015; TUVE', Cristina/P-3933-2015; KIM, Tae Jeong/P-7848-2015; Arce, Pedro/L-1268-2014; Flix, Josep/G-5414-2012; Azarkin, Maxim/N-2578-2015; Paganoni, Marco/A-4235-2016; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Leonidov, Andrey/P-3197-2014; Bernardes, Cesar Augusto/D-2408-2015; Lazzizzera, Ignazio/E-9678-2015; Sen, Sercan/C-6473-2014; vilar, rocio/P-8480-2014; D'Alessandro, Raffaello/F-5897-2015; Belyaev, Alexander/F-6637-2015; Stahl, Achim/E-8846-2011; Trocsanyi, Zoltan/A-5598-2009; Konecki, Marcin/G-4164-2015; Bedoya, Cristina/K-8066-2014; My, Salvatore/I-5160-2015; Rovelli, Tiziano/K-4432-2015 OI Scodellaro, Luca/0000-0002-4974-8330; Calvo Alamillo, Enrique/0000-0002-1100-2963; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Marinho, Franciole/0000-0002-7327-0349; Ferguson, Thomas/0000-0001-5822-3731; Benussi, Luigi/0000-0002-2363-8889; Dahms, Torsten/0000-0003-4274-5476; Grandi, Claudio/0000-0001-5998-3070; Dogangun, Oktay/0000-0002-1255-2211; de Jesus Damiao, Dilson/0000-0002-3769-1680; Codispoti, Giuseppe/0000-0003-0217-7021; Cerrada, Marcos/0000-0003-0112-1691; Azzi, Patrizia/0000-0002-3129-828X; Rolandi, Luigi (Gigi)/0000-0002-0635-274X; Montanari, Alessandro/0000-0003-2748-6373; Tomei, Thiago/0000-0002-1809-5226; Ivanov, Andrew/0000-0002-9270-5643; Hill, Christopher/0000-0003-0059-0779; Wimpenny, Stephen/0000-0003-0505-4908; Mundim, Luiz/0000-0001-9964-7805; De La Cruz Burelo, Eduard/0000-0002-7469-6974; Tinoco Mendes, Andre David/0000-0001-5854-7699; Novaes, Sergio/0000-0003-0471-8549; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Della Ricca, Giuseppe/0000-0003-2831-6982; Seixas, Joao/0000-0002-7531-0842; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Gerbaudo, Davide/0000-0002-4463-0878; Matorras, Francisco/0000-0003-4295-5668; TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; Arce, Pedro/0000-0003-3009-0484; Flix, Josep/0000-0003-2688-8047; Paganoni, Marco/0000-0003-2461-275X; Gulmez, Erhan/0000-0002-6353-518X; Lazzizzera, Ignazio/0000-0001-5092-7531; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Belyaev, Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279; Konecki, Marcin/0000-0001-9482-4841; Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680; Rovelli, Tiziano/0000-0002-9746-4842 FU BMWF (Austria); FWF (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MES (Bulgaria); CERN; CAS (China); MoST (China); NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); MoER (Estonia) [SF0690030s09]; ERDF (Estonia); Academy of Finland (Finland); MEC (Finland); HIP (Finland); CEA (France); CNRS/IN2P3 (France); BMBF (Germany); DFG (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NKTH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF (Korea); WCU (Korea); LAS (Lithuania); CINVESTAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); MSI (New Zealand); PAEC (Pakistan); MSHE (Poland); NSC (Poland); FCT (Portugal); JINR (Armenia); JINR (Belarus); JINR (Georgia); JINR (Ukraine); JINR (Uzbekistan); MON (Russia); RosAtom (Russia); RAS (Russia); RFBR (Russia); MSTD (Serbia); SEIDI (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); ThEP (Thailand); IPST (Thailand); NECTEC (Thailand); TUBITAK (Turkey); TAEK (Turkey); NASU (Ukraine); STFC (United Kingdom); DOE (USA); NSF (USA); Marie-Curie programme (European Union); European Research Council (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Austrian Science Fund (FWF); Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of Czech Republic; Council of Science and Industrial Research, India; Compagnia di San Paolo (Torino); HOMING PLUS programme of Foundation for Polish Science; European Union, Regional Development Fund FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC machine. We thank the technical and administrative staff at CERN and other CMS institutes, and acknowledge support from BMWF and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); MoER, SF0690030s09 and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NKTH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF and WCU (Korea); LAS (Lithuania); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MSI (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Armenia, Belarus, Georgia, Ukraine, Uzbekistan); MON, RosAtom, RAS and RFBR (Russia); MSTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); ThEP, IPST and NECTEC (Thailand); TUBITAK and TAEK (Turkey); NASU (Ukraine); STFC (United Kingdom); DOE and NSF (USA).; Individuals have received support from the Marie-Curie programme and the European Research Council (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Austrian Science Fund (FWF); the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of Czech Republic; the Council of Science and Industrial Research, India; the Compagnia di San Paolo (Torino); and the HOMING PLUS programme of Foundation for Polish Science, cofinanced from European Union, Regional Development Fund. NR 51 TC 1 Z9 1 U1 1 U2 73 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD NOV PY 2012 IS 11 AR 088 DI 10.1007/JHEP11(2012)088 PG 34 WC Physics, Particles & Fields SC Physics GA 052LG UT WOS:000312198500023 ER PT J AU Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Aguilo, E Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hammer, J Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Pernicka, M Rahbaran, B Rohringer, C Rohringer, H Schofbeck, R Strauss, J Taurok, A Waltenberger, W Walzel, G Widl, E Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Bansal, S Cornelis, T De Wolf, EA Janssen, X Luyckx, S Mucibello, L Ochesanu, S Roland, B Rougny, R Selvaggi, M Staykova, Z Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Suarez, RG Kalogeropoulos, A Maes, M Olbrechts, A Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Clerbaux, B De Lentdecker, G Dero, V Gay, APR Hreus, T Leonard, A Marage, PE Reis, T Thomas, L Vander 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CA CMS Collaboration TI Measurement of the t(t)over-bar production cross section in the dilepton channel in pp collisions at root s=7 TeV SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering ID PROTON-PROTON COLLISIONS; QUARK PAIR PRODUCTION; TOP-QUARK; ATLAS DETECTOR; GAUGE COUPLINGS; LIMITS; BOSON; LHC AB The t (t) over bar production cross section (sigma(t (t) over bar)) is measured in proton-proton collisions at root s = 7 TeV in data collected by the CMS experiment, corresponding to an integrated luminosity of 2.3 fb(-1). The measurement is performed in events with two leptons (electrons or muons) in the final state, at least two jets identified as jets originating from b quarks, and the presence of an imbalance in transverse momentum. The measured value of sigma(t (t) over bar) for a top-quark mass of 172.5 GeV is 161.9 +/- 2.5 (stat.)(-5.0)(+5.1) (syst.) +/- 3.6 (lumi.) pb, consistent with the prediction of the standard model. 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[Anjos, T. S.; Bernardes, C. A.; Gregores, E. M.; Mercadante, P. G.] Univ Fed ABC, Santo Andre, Brazil. [Dias, F. A.; Dubinin, M.; Apresyan, A.; Bornheim, A.; Chen, Y.; Di Marco, E.; Duarte, J.; Gataullin, M.; Ma, Y.; Mott, A.; Newman, H. B.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Veverka, J.; Wilkinson, R.; Yang, Y.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Genchev, V.; Iaydjiev, P.; Puljak, I.; Chierici, R.; Sharma, A.; Mohanty, A. K.; Calabria, C.; De Filippis, N.; Masetti, G.; Tropiano, A.; Benaglia, A.; Di Matteo, L.; Gennai, S.; Massironi, A.; De Cosa, A.; Paolucci, P.; Bacchetta, N.; Branca, A.; Tosi, M.; Lucaroni, A.; Taroni, S.; Fiori, F.; Squillacioti, P.; Tonelli, G.; Venturi, A.; Del Re, D.; Grassi, M.; Meridiani, P.; Kossov, M.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Baillon, P.; Ball, A. H.; Barney, D.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Coarasa Perez, J. A.; D'Enterria, D.; Dabrowski, A.; De Roeck, A.; Di Guida, S.; Dobson, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Frisch, B.; Funk, W.; Georgiou, G.; Giffels, M.; Gigi, D.; Gill, K.; Giordano, D.; Giunta, M.; Glege, F.; Gomez-Reino Garrido, R.; Govoni, P.; Gowdy, S.; Guida, R.; Hansen, M.; Harris, P.; Hartl, C.; Harvey, J.; Hegner, B.; Hinzmann, A.; Innocente, V.; Janot, P.; Kaadze, K.; Karavakis, E.; Kousouris, K.; Lecoq, P.; Lee, Y. -J.; Lenzi, P.; Lourenco, C.; Maeki, T.; Malberti, M.; Malgeri, L.; Mannelli, M.; Meijers, F.; Mersi, S.; Meschi, E.; Moser, R.; Mozer, M. U.; Mulders, M.; Musella, P.; Nesvold, E.; Orimoto, T.; Orsini, L.; Palencia Cortezon, E.; Perez, E.; Perrozzi, L.; Petrilli, A.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Piparo, D.; Polese, G.; Quertenmont, L.; Racz, A.; Reece, W.; Antunes, J. Rodrigues; Rolandi, G.; Rommerskirchen, T.; Rovelli, C.; Rovere, M.; Sakulin, H.; Santanastasio, F.; Schaefer, C.; Schwick, C.; Segoni, I.; Sekmen, S.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Tsirou, A.; Veres, G. I.; Vlimant, J. R.; Woehri, H. K.; Worm, S. D.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Plestina, R.; Baffioni, S.; Beaudette, F.; Benhabib, L.; Bianchini, L.; Bluj, M.; Broutin, C.; Busson, P.; Charlot, C.; Daci, N.; Dahms, T.; Dobrzynski, L.; de Cassagnac, R. Granier; Haguenauer, M.; Mine, P.; Mironov, C.; Naranjo, I. N.; Nguyen, M.; Ochando, C.; Paganini, P.; Sabes, D.; Salerno, R.; Sirois, Y.; Veelken, C.; Zabi, A.; Guthoff, M.; Hauth, T.; Foudas, C.; Hajdu, C.] Ecole Polytech, Lab Leprince Ringuet, IN2P3, CNRS, Palaiseau, France. [Assran, Y.] Suez Canal Univ, Suez, Egypt. [Elgammal, S.; Khalil, S.] Zewail City Sci & Technol, Zewail, Egypt. [Kamel, A. Ellithi] Cairo Univ, Cairo, Egypt. [Mahmoud, M. A.] Fayoum Univ, Al Fayyum, Egypt. [Radi, A.] British Univ, Cairo, Egypt. [Bluj, M.] Natl Ctr Nucl Res, Otwock, Poland. [Agram, J. -L.; Conte, E.; Drouhin, F.; Fontaine, J. -C.] Univ Haute Alsace, Mulhouse, France. [Zhukov, V.] Moscow MV Lomonosov State Univ, Moscow, Russia. [Banzuzi, K.; Karjalainen, A.; Korpela, A.; Tuuva, T.] Lappeenranta Univ Technol, Lappeenranta, Finland. [Besancon, M.; Choudhury, S.; Dejardin, M.; Denegri, D.; Fabbro, B.; Faure, J. L.; Ferri, F.; Ganjour, S.; Givernaud, A.; Gras, P.; de Monchenault, G. Hamel; Jarry, P.; Locci, E.; Malcles, J.; Millischer, L.; Nayak, A.; Rander, J.; Rosowsky, A.; Shreyber, I.; Titov, M.] CEA Saclay, DSM IRFU, F-91191 Gif Sur Yvette, France. [Agram, J. -L.; Andrea, J.; Bloch, D.; Bodin, D.; Brom, J. -M.; Cardaci, M.; Chabert, E. C.; Collard, C.; Conte, E.; Drouhin, F.; Ferro, C.; Fontaine, J. -C.; Gele, D.; Goerlach, U.; Juillot, P.; Le Bihan, A. -C.; Van Hove, P.] Univ Haute Alsace Mulhouse, Inst Pluridisciplinaire Hubert Curien, Univ Strasbourg, CNRS,IN2P3, Strasbourg, France. [Fassi, F.; Mercier, D.] Inst Natl Phys Nucl & Phys Particules, Ctr Calcul, CNRS, IN2P3, Villeurbanne, France. [Beauceron, S.; Beaupere, N.; Bondu, O.; Boudoul, G.; Chasserat, J.; Chierici, R.; Contardo, D.; Depasse, P.; El Mamouni, H.; Fay, J.; Gascon, S.; Gouzevitch, M.; Ille, B.; Kurca, T.; Lethuillier, M.; Mirabito, L.; Perries, S.; Sordini, V.; Tschudi, Y.; Verdier, P.; Viret, S.] Univ Lyon 1, CNRS, Univ Lyon, IN2P3,Inst Phys Nucl Lyon, F-69622 Villeurbanne, France. [Tsamalaidze, Z.] Tbilisi State Univ, Inst High Energy Phys & Informatizat, GE-380086 Tbilisi, Rep of Georgia. [Klein, B.; Anagnostou, G.; Beranek, S.; Edelhoff, M.; Feld, L.; Heracleous, N.; Hindrichs, O.; Jussen, R.; Merz, J.; Ostapchuk, A.; Perieanu, A.; Raupach, F.; Sammet, J.; Schael, S.; Sprenger, D.; Weber, H.; Wittmer, B.; Zhukov, V.] Rhein Westfal TH Aachen, Phys Inst 1, Aachen, Germany. [Ata, M.; Caudron, J.; Dietz-Laursonn, E.; Duchardt, D.; Erdmann, M.; Fischer, R.; Gueth, A.; Hebbeker, T.; Heidemann, C.; Hoepfner, K.; Klingebiel, D.; Kreuzer, P.; Magass, C.; Merschmeyer, M.; Meyer, A.; Olschewski, M.; Papacz, P.; Pieta, H.; Reithler, H.; Schmitz, S. A.; Sonnenschein, L.; Steggemann, J.; Teyssier, D.; Weber, M.] Rhein Westfal TH Aachen, Phys Inst A3, Aachen, Germany. [Bontenackels, M.; Cherepanov, V.; Fluegge, G.; Geenen, H.; Geisler, M.; Ahmad, W. Haj; Hoehle, F.; Kargoll, B.; Kress, T.; Kuessel, Y.; Nowack, A.; Perchalla, L.; Pooth, O.; Sauerland, P.; Stahl, A.] Rhein Westfal TH Aachen, Phys Inst B3, Aachen, Germany. [Bergholz, M.; Lohmann, W.; Schmidt, R.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Horvath, D.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Bergholz, M.; Lohmann, W.; Schmidt, R.] Eotvos Lorand Univ, Budapest, Hungary. [Guchait, M.] Tata Inst Fundamental Res HECR, Bombay, Maharashtra, India. [Thyssen, F.; Martin, M. Aldaya; Behr, J.; Behrenhoff, W.; Behrens, U.; Bergholz, M.; Bethani, A.; Borras, K.; Burgmeier, A.; Cakir, A.; Calligaris, L.; Campbell, A.; Castro, E.; Costanza, F.; Dammann, D.; Pardos, C. Diez; Eckerlin, G.; Eckstein, D.; Flucke, G.; Geiser, A.; Glushkov, I.; Gunnellini, P.; Habib, S.; Hauk, J.; Hellwig, G.; Jung, H.; Kasemann, M.; Katsas, P.; Kleinwort, C.; Kluge, H.; Knutsson, A.; Kraemer, M.; Kruecker, D.; Kuznetsova, E.; Lange, W.; Lohmann, W.; Lutz, B.; Mankel, R.; Marfin, I.; Marienfeld, M.; Melzer-Pellmann, I. -A.; Meyer, A. B.; Mnich, J.; Mussgiller, A.; Naumann-Emme, S.; Olzem, J.; Perrey, H.; Petrukhin, A.; Pitzl, D.; Raspereza, A.; Cipriano, P. M. Ribeiro; Riedl, C.; Ron, E.; Rosin, M.; Salfeld-Nebgen, J.; Schmidt, R.; Schoerner-Sadenius, T.; Spiridonov, A.; Stein, M.; Walsh, R.; Wissing, C.] DESY, Hamburg, Germany. [Autermann, C.; Blobel, V.; Draeger, J.; Enderle, H.; Erfle, J.; Gebbert, U.; Goerner, M.; Hermanns, T.; Hoeing, R. S.; Kaschube, K.; Kaussen, G.; Kirschenmann, H.; Klanner, R.; Lange, J.; Mura, B.; Nowak, F.; Peiffer, T.; Pietsch, N.; Rathjens, D.; Sander, C.; Schettler, H.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Schroeder, M.; Schum, T.; Seidel, M.; Sola, V.; Stadie, H.; Steinbrueck, G.; Thomsen, J.; Vanelderen, L.] Univ Hamburg, Hamburg, Germany. [Barth, C.; Berger, J.; Boeser, C.; Chwalek, T.; De Boer, W.; Descroix, A.; Dierlamm, A.; Feindt, M.; Guthoff, M.; Hackstein, C.; Hartmann, F.; Hauth, T.; Heinrich, M.; Held, H.; Hoffmann, K. H.; Honc, S.; Katkov, I.; Komaragiri, J. R.; Pardo, P. Lobelle; Martschei, D.; Mueller, S.; Mueller, Th.; Niegel, M.; Nuernberg, A.; Oberst, O.; Oehler, A.; Ott, J.; Quast, G.; Rabbertz, K.; Ratnikov, F.; Ratnikova, N.; Roecker, S.; Scheurer, A.; Schilling, F. -P.; Schott, G.; Simonis, H. J.; Stober, F. M.; Troendle, D.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weiler, T.; Zeise, M.] Univ Karlsruhe, Inst Expt Kernphys, D-7500 Karlsruhe, Germany. [Attikis, A.; Mavromanolakis, G.; Daskalakis, G.; Geralis, T.; Kesisoglou, S.; Kyriakis, A.; Loukas, D.; Markou, A.; Markou, C.; Mavrommatis, C.; Ntomari, E.] Inst Nucl Phys Demokritos, Aghia Paraskevi, Greece. [Gouskos, L.; Mertzimekis, T. J.; Panagiotou, A.; Saoulidou, N.] Univ Athens, Athens, Greece. [Evangelou, I.; Foudas, C.; Kokkas, P.; Manthos, N.; Papadopoulos, I.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.] KFKI Res Inst Particle & Nucl Phys, Budapest, Hungary. [Beni, N.; Czellar, S.; Molnar, J.; Palinkas, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Karancsi, J.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, H-4012 Debrecen, Hungary. [Beri, S. B.; Bhatnagar, V.; Dhingra, N.; Gupta, R.; Jindal, M.; Kaur, M.; Mehta, M. Z.; Nishu, N.; Saini, L. K.; Sharma, A.; Singh, J.] Panjab Univ, Chandigarh 160014, India. [Kumar, Ashok; Kumar, Arun; Ahuja, S.; Bhardwaj, A.; Choudhary, B. C.; Malhotra, S.; Naimuddin, M.; Ranjan, K.; Sharma, V.; Shivpuri, R. K.] Univ Delhi, Delhi 110007, India. [Banerjee, S.; Bhattacharya, S.; Dutta, S.; Gomber, B.; Jain, Sa.; Jain, Sh.; Khurana, R.; Sarkar, S.; Sharan, M.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Choudhury, R. K.; Dutta, D.; Kailas, S.; Kumar, V.; Mehta, P.; Mohanty, A. K.; Pant, L. M.; Shukla, P.] Bhabha Atom Res Ctr, Bombay 400085, Maharashtra, India. [Aziz, T.; Ganguly, S.; Guchait, M.; Maity, M.; Majumder, G.; Mazumdar, K.; Mohanty, G. B.; Parida, B.; Sudhakar, K.; Wickramage, N.] Tata Inst Fundamental Res EHEP, Bombay, Maharashtra, India. [Banerjee, S.; Dugad, S.] Tata Inst Fundamental Res HECR, Bombay, Maharashtra, India. [Maity, M.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Bakhshiansohi, H.; Fahim, A.; Jafari, A.] Sharif Univ Technol, Tehran, Iran. [Etesami, S. M.; Zeinali, M.] Isfahan Univ Technol, Esfahan, Iran. [Safarzadeh, B.] Islamic Azad Univ, Sci & Res Branch, Plasma Phys Res Ctr, Tehran, Iran. [Colafranceschi, S.] Univ Rome, Fac Ingn, Rome, Italy. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; Colaleo, A.; Creanza, D.; De Filippis, N.; De Palma, M.; Iaselli, G.; Lusito, L.; Maggi, G.; Maggi, M.; Marangelli, B.; My, S.; Nuzzo, S.; Pacifico, N.; Pompili, A.; Pugliese, G.; Selvaggi, G.; Silvestris, L.; Singh, G.; Zito, G.] INFN Sez Bari, Bari, Italy. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; De Palma, M.; Lusito, L.; Marangelli, B.; Nuzzo, S.; Pacifico, N.; Pompili, A.; Selvaggi, G.; Singh, G.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Meneghelli, M.; Montanari, A.; Navarria, F. L.; Odorici, F.; Perrotta, A.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G.; Travaglini, R.] INFN Sez Bologna, Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Capiluppi, P.; Castro, A.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Meneghelli, M.; Navarria, F. L.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] INFN Sez Catania, Catania, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gallo, E.; Gonzi, S.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] INFN Sez Firenze, Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gonzi, S.] Univ Florence, Florence, Italy. [Fabbri, F.; Benussi, L.; Bianco, S.; Colafranceschi, S.; Piccolo, D.] INFN Lab Nazl Frascati, Frascati, Italy. [Fabbricatore, P.; Musenich, R.] INFN Sez Genova, Genoa, Italy. Univ Genoa, Genoa, Italy. [Benaglia, A.; De Guio, F.; Di Matteo, L.; Fiorendi, S.; Gennai, S.; Ghezzi, A.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Massironi, A.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; Sala, S.; de Fatis, T. Tabarelli] INFN Sez Milano Bicocca, Milan, Italy. [Benaglia, A.; De Guio, F.; Di Matteo, L.; Fiorendi, S.; Ghezzi, A.; Manzoni, R. A.; Martelli, A.; Massironi, A.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Montoya, C. A. Carrillo; Cavallo, N.; De Cosa, A.; Dogangun, O.; Fabozzi, F.; Iorio, A. O. M.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.] INFN Sez Napoli, Naples, Italy. [De Cosa, A.; Dogangun, O.; Merola, M.] Univ Naples Federico II, Naples, Italy. [Azzi, P.; Bacchetta, N.; Bisello, D.; Branca, A.; Carlin, R.; Checchia, P.; Dorigo, T.; Gasparini, F.; Gasparini, U.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Lazzizzera, I.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Triossi, A.; Vanini, S.; Zotto, P.; Zumerle, G.] INFN Sez Padova, Padua, Italy. [Bisello, D.; Carlin, R.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Vanini, S.; Zotto, P.] Univ Padua, Padua, Italy. [Kanishchev, K.; Lazzizzera, I.] Univ Trento Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Torre, P.; Vitulo, P.] INFN Sez Pavia, Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Torre, P.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Fano, L.; Lariccia, P.; Lucaroni, A.; Mantovani, G.; Menichelli, M.; Nappi, A.; Romeo, F.; Saha, A.; Santocchia, A.; Spiezia, A.; Taroni, S.] INFN Sez Perugia, Perugia, Italy. [Biasini, M.; Fano, L.; Lariccia, P.; Lucaroni, A.; Mantovani, G.; Nappi, A.; Romeo, F.; Santocchia, A.; Spiezia, A.; Taroni, S.] Univ Perugia, I-06100 Perugia, Italy. [Azzurri, P.; Bagliesi, G.; Boccali, T.; Broccolo, G.; Castaldi, R.; D'Agnolo, R. T.; Dell'Orso, R.; Fiori, F.; Foa, L.; Giassi, A.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] INFN Sez Pisa, Pisa, Italy. [Fiori, F.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Azzurri, P.; Broccolo, G.; D'Agnolo, R. T.; Foa, L.; Ligabue, F.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Diemoz, M.; Grassi, M.; Longo, E.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Sigamani, M.; Soffi, L.] INFN Sez Roma, Rome, Italy. [Barone, L.; Del Re, D.; Grassi, M.; Longo, E.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Soffi, L.] Univ Roma La Sapienza, Rome, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata, Potenza, Italy. [Meola, S.] Univ Guglielmo Marconi, Rome, Italy. [Martini, L.] Univ Siena, I-53100 Siena, Italy. [Serban, A. T.] Univ Bucharest, Fac Phys, Bucharest, Romania. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Biino, C.; Cartiglia, N.; Costa, M.; Dattola, D.; Demaria, N.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Pastrone, N.; Pelliccioni, M.; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.; Staiano, A.; Pereira, A. Vilela] INFN Sez Torino, Turin, Italy. [Amapane, N.; Argiro, S.; Costa, M.; Migliore, E.; Monaco, V.; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Migliore, E.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; Marone, M.; Montanino, D.; Penzo, A.; Schizzi, A.] INFN Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; Marone, M.; Montanino, D.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Heo, S. G.; Kim, T. Y.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Chang, S.; Kim, D. H.; Kim, G. N.; Kong, D. J.; Park, H.; Ro, S. R.; Son, D. C.; Son, T.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, J. Y.; Kim, Zero J.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, T. J.; Lee, K. S.; Moon, D. H.; Park, S. K.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Cho, Y.; Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. S.; Kwon, E.; Lee, B.; Lee, J.; Lee, S.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Bilinskas, M. J.; Grigelionis, I.; Janulis, M.; Juodagalvis, A.] Vilnius State Univ, Vilnius, Lithuania. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Lopez-Fernandez, R.; Magana Villalba, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] Ctr Invest & Estudios Avanzados IPN, Mexico City, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.; Reyes-Santos, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Bell, A. J.; Butler, P. H.; Doesburg, R.; Reucroft, S.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Asghar, M. I.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Boimska, B.; Frueboes, T.; Gokieli, R.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Almeida, N.; Bargassa, P.; David, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Belotelov, I.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Kozlov, G.; Lanev, A.; Malakhov, A.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Smirnov, V.; Volodko, A.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Smirnov, V.; Evstyukhin, S.; Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Matveev, V.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Russian Acad Sci, Inst Nucl Res, Moscow, Russia. [Epshteyn, V.; Erofeeva, M.; Gavrilov, V.; Kossov, M.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Stolin, V.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Belyaev, A.; Boos, E.; Bunichev, V.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Markina, A.; Obraztsov, S.; Perfilov, M.; Popov, A.; Sarycheva, L.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Volodko, A.; Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Grishin, V.; Kachanov, V.; Konstantinov, D.; Korablev, A.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.] Univ Belgrade, Fac Phys, YU-11001 Belgrade, Serbia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Alcaraz Maestre, J.; Arce, P.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.; Willmott, C.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain. [Albajar, C.; Codispoti, G.; de Troconiz, J. F.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.; Piedra Gomez, J.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Chuang, S. H.; Duarte Campderros, J.; Felcini, M.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Graziano, A.; Jorda, C.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Sobron Sanudo, M.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Bertl, W.; Deiters, K.; Erdmann, W.; Gabathuler, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Meier, F.; Renker, D.; Rohe, T.; Sibille, J.] Paul Scherrer Inst, Villigen, Switzerland. [Baeni, L.; Bortignon, P.; Buchmann, M. A.; Casal, B.; Chanon, N.; Deisher, A.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eugster, J.; Freudenreich, K.; Grab, C.; Hits, D.; Lecomte, P.; Lustermann, W.; Marini, A. C.; del Arbol, P. Martinez Ruiz; Mohr, N.; Moortgat, F.; Naegeli, C.; Nef, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pape, L.; Pauss, F.; Peruzzi, M.; Ronga, F. J.; Rossini, M.; Sala, L.; Sanchez, A. K.; Starodumov, A.; Stieger, B.; Takahashi, M.; Tauscher, L.; Thea, A.; Theofilatos, K.; Treille, D.; Urscheler, C.; Wallny, R.; Weber, H. A.; Wehrli, L.] Swiss Fed Inst Technol, Inst Particle Phys, Zurich, Switzerland. [Amsler, C.; Chiochia, V.; De Visscher, S.; Favaro, C.; Rikova, M. Ivova; Mejias, B. Millan; Otiougova, P.; Robmann, P.; Snoek, H.; Tupputi, S.; Verzetti, M.] Univ Zurich, Zurich, Switzerland. [Chang, Y. H.; Chen, K. H.; Kuo, C. M.; Li, S. W.; Lin, W.; Liu, Z. K.; Lu, Y. J.; Mekterovic, D.; Singh, A. P.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Majumder, G.; Chang, Y. H.; Bartalini, P.; Chang, P.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Dietz, C.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wan, X.; Wang, M.] Natl Taiwan Univ NTU, Taipei, Taiwan. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Karaman, T.; Karapinar, G.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, L. N.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Yildirim, E.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey. [Cankocak, K.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Bostock, F.; Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Kreczko, L.; Metson, S.; Newbold, D. M.; Nirunpong, K.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Belyaev, A.; Basso, L.; Bell, K. W.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Jackson, J.; Kennedy, B. W.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Womersley, W. J.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Bainbridge, R.; Ball, G.; Beuselinck, R.; Buchmuller, O.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Papageorgiou, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Ryan, M. J.; Seez, C.; Sharp, P.; Sparrow, A.; Stoye, M.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.; Whyntie, T.] Univ London Imperial Coll Sci Technol & Med, London, England. [Chadwick, M.; Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Hatakeyama, K.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; John, J. St.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Bhattacharya, S.; Alimena, J.; Cutts, D.; Ferapontov, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Nguyen, D.; Segala, M.; Sinthuprasith, T.; Speer, T.; Tsang, K. V.] Brown Univ, Providence, RI 02912 USA. [Roland, B.; Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Dolen, J.; Erbacher, R.; Gardner, M.; Houtz, R.; Ko, W.; Kopecky, A.; Miceli, T.; Pellett, D.; Ricci-tam, F.; Rutherford, B.; Searle, M.; Smith, J.; Squires, M.; Tripathi, M.; Sierra, R. Vasquez] Univ Calif Davis, Davis, CA 95616 USA. [Weber, H.; Andreev, V.; Cline, D.; Cousins, R.; Duris, J.; Erhan, S.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Plager, C.; Rakness, G.; Schlein, P.; Traczyk, P.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Liu, H.; Babb, J.; Clare, R.; Dinardo, M. E.; Ellison, J.; Gary, J. W.; Giordano, F.; Hanson, G.; Jeng, G. Y.; Long, O. R.; Luthra, A.; Nguyen, H.; Paramesvaran, S.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sharma, V.; Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; Evans, D.; Golf, F.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Macneill, I.; Mangano, B.; Padhi, S.; Palmer, C.; Petrucciani, G.; Pieri, M.; Sani, M.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuethwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bellan, R.; Campagnari, C.; D'Alfonso, M.; Danielson, T.; Flowers, K.; Geffert, P.; Incandela, J.; Justus, C.; Kalavase, P.; Koay, S. A.; Kovalskyi, D.; Krutelyov, V.; Lowette, S.; Mccoll, N.; Pavlunin, V.; Rebassoo, F.; Ribnik, J.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Akgun, B.; Azzolini, V.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Liu, Y. F.; Paulini, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Edelmaier, C. J.; Ford, W. T.; Gaz, A.; Heyburn, B.; Lopez, E. Luiggi; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Eggert, N.; Gibbons, L. K.; Heltsley, B.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Vaughan, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bloch, I.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Green, D.; Gutsche, O.; Hanlon, J.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Kilminster, B.; Klima, B.; Kunori, S.; Kwan, S.; Leonidopoulos, C.; Linacre, J.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Tan, P.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Wu, W.; Yang, F.; Yumiceva, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Chen, M.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Drozdetskiy, A.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Gartner, J.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Remington, R.; Rinkevicius, A.; Sellers, P.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Hewamanage, S.; Lebolo, L. M.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Gleyzer, S. V.; Haas, J.; Hagopian, S.; Hagopian, V.; Jenkins, M.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Vodopiyanov, I.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Anghel, I. M.; Apanasevich, L.; Bai, Y.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Callner, J.; Cavanaugh, R.; Dragoiu, C.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Lacroix, F.; Malek, M.; O'Brien, C.; Silkworth, C.; Strom, D.; Varelas, N.] Univ Illinois Chicago UIC, Chicago, IL USA. [Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Duru, F.; Griffiths, S.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Newsom, C. R.; Norbeck, E.; Onel, Y.; Ozok, F.; Sen, S.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Giurgiu, G.; Gritsan, A. V.; Guo, Z. J.; Hu, G.; Maksimovic, P.; Rappoccio, S.; Swartz, M.; Whitbeck, A.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Grachov, O.; Iii, R. P. Kenny; Murray, M.; Noonan, D.; Sanders, S.; Stringer, R.; Tinti, G.; Wood, J. S.; Zhukova, V.] Univ Kansas, Lawrence, KS 66045 USA. [Khalil, S.; Barfuss, A. F.; Bolton, T.; Chakaberia, I.; Ivanov, A.; Makouski, M.; Maravin, Y.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Boutemeur, M.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kirn, M.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Peterman, A.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.; Twedt, E.] Univ Maryland, College Pk, MD 20742 USA. [Li, W.; Dutta, D.; Apyan, A.; Bauer, G.; Bendavid, J.; Busza, W.; Butz, E.; Cali, I. A.; Chan, M.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Hahn, K. A.; Kim, Y.; Klute, M.; Krajczar, K.; Luckey, P. D.; Ma, T.; Nahn, S.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Rudolph, M.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Sung, K.; Velicanu, D.; Wenger, E. A.; Wolf, R.; Wyslouch, B.; Xie, S.; Yang, M.; Yilmaz, Y.; Yoon, A. S.; Zanetti, M.] MIT, Cambridge, MA 02139 USA. [Cooper, S. I.; Dahmes, B.; De Benedetti, A.; Franzoni, G.; Gude, A.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Sasseville, M.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Cremaldi, L. M.; Kroeger, R.; Perera, L.; Rahmat, R.; Sanders, D. A.] Univ Mississippi, University, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Butt, J.; Claes, D. R.; Dominguez, A.; Eads, M.; Keller, J.; Kravchenko, I.; Lazo-Flores, J.; Malbouisson, H.; Malik, S.; Snow, G. R.] Univ Nebraska Lincoln, Lincoln, NE USA. [Baur, U.; Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Kumar, A.; Shipkowski, S. P.; Smith, K.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Nash, D.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Anastassov, A.; Kubik, A.; Mucia, N.; Odell, N.; Ofierzynski, R. A.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Antonelli, L.; Berry, D.; Brinkerhoff, A.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kolb, J.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Morse, D. M.; Pearson, T.; Ruchti, R.; Slaunwhite, J.; Valls, N.; Wayne, M.; Wolf, M.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Bylsma, B.; Durkin, L. S.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Puigh, D.; Rodenburg, M.; Vuosalo, C.; Williams, G.; Winer, B. L.] Ohio State Univ, Columbus, OH 43210 USA. [Adam, N.; Berry, E.; Elmer, P.; Gerbaudo, D.; Halyo, V.; Hebda, P.; Hegeman, J.; Hunt, A.; Jindal, P.; Pegna, D. Lopes; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Raval, A.; Safdi, B.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Acosta, J. G.; Brownson, E.; Huang, X. T.; Lopez, A.; Mendez, H.; Oliveros, S.; Vargas, J. E. Ramirez; Zatserklyaniy, A.] Univ Puerto Rico, Mayaguez, PR USA. [Alagoz, E.; Barnes, V. E.; Benedetti, D.; Bolla, G.; Bortoletto, D.; De Mattia, M.; Everett, A.; Hu, Z.; Jones, M.; Koybasi, O.; Kress, M.; Laasanen, A. T.; Leonardo, N.; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Marono, M. Vidal; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Guragain, S.; Parashar, N.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Boulahouache, C.; Ecklund, K. M.; Geurts, F. J. M.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; Chung, Y. S.; Covarelli, R.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Miner, D. C.; Vishnevskiy, D.; Zielinski, M.] Univ Rochester, Rochester, NY 14627 USA. [Malik, S.; Bhatti, A.; Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Lath, A.; Panwalkar, S.; Park, M.; Patel, R.; Rekovic, V.; Robles, J.; Rose, K.; Salur, S.; Schnetzer, S.; Seitz, C.; Somalwar, S.; Stone, R.; Thomas, S.] Rutgers State Univ, Piscataway, NJ USA. [Cerizza, G.; Hollingsworth, M.; Spanier, S.; Yang, Z. C.; York, A.] Univ Tennessee, Knoxville, TN USA. [Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Khotilovich, V.; Montalvo, R.; Osipenkov, I.; Pakhotin, Y.; Roe, J.; Safonov, A.; Sakuma, T.; Sengupta, S.; Suarez, I.; Tatarinov, A.; Toback, D.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Damgov, J.; Dudero, P. R.; Jeong, C.; Kovitanggoon, K.; Lee, S. W.; Libeiro, T.; Roh, Y.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Appelt, E.; Delannoy, A. G.; Florez, C.; Greene, S.; Gurrola, A.; Johns, W.; Johnston, C.; Kurt, P.; Maguire, C.; Melo, A.; Sharma, M.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN USA. [Arenton, M. W.; Balazs, M.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Lin, C.; Neu, C.; Wood, J.; Yohay, R.] Univ Virginia, Charlottesville, VA USA. [Gollapinni, S.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sakharov, A.] Wayne State Univ, Detroit, MI USA. [Anderson, M.; Bachtis, M.; Belknap, D.; Borrello, L.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Friis, E.; Gray, L.; Grogg, K. S.; Grothe, M.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Klukas, J.; Lanaro, A.; Lazaridis, C.; Leonard, J.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Palmonari, F.; Pierro, G. A.; Ross, I.; Savin, A.; Smith, W. H.; Swanson, J.] Univ Wisconsin, Madison, WI 53706 USA. RP Chatrchyan, S (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Sznajder, Andre/L-1621-2016; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Gerbaudo, Davide/J-4536-2012; Andreev, Vladimir/M-8665-2015; TUVE', Cristina/P-3933-2015; KIM, Tae Jeong/P-7848-2015; Arce, Pedro/L-1268-2014; Flix, Josep/G-5414-2012; Della Ricca, Giuseppe/B-6826-2013; Azarkin, Maxim/N-2578-2015; Paganoni, Marco/A-4235-2016; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Seixas, Joao/F-5441-2013; Vilela Pereira, Antonio/L-4142-2016; Sen, Sercan/C-6473-2014; D'Alessandro, Raffaello/F-5897-2015; Belyaev, Alexander/F-6637-2015; Stahl, Achim/E-8846-2011; Trocsanyi, Zoltan/A-5598-2009; Konecki, Marcin/G-4164-2015; Bedoya, Cristina/K-8066-2014; My, Salvatore/I-5160-2015; Matorras, Francisco/I-4983-2015; Ragazzi, Stefano/D-2463-2009; Dremin, Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Leonidov, Andrey/M-4440-2013; Scodellaro, Luca/K-9091-2014; Josa, Isabel/K-5184-2014; Calvo Alamillo, Enrique/L-1203-2014; Paulini, Manfred/N-7794-2014; Vogel, Helmut/N-8882-2014; Marinho, Franciole/N-8101-2014; Ferguson, Thomas/O-3444-2014; Benussi, Luigi/O-9684-2014; Dahms, Torsten/A-8453-2015; Grandi, Claudio/B-5654-2015; Leonidov, Andrey/P-3197-2014; Bernardes, Cesar Augusto/D-2408-2015; Lazzizzera, Ignazio/E-9678-2015; Dogangun, Oktay/L-9252-2013; Marlow, Daniel/C-9132-2014; Oguri, Vitor/B-5403-2013; Janssen, Xavier/E-1915-2013; Novaes, Sergio/D-3532-2012; Bartalini, Paolo/E-2512-2014; Codispoti, Giuseppe/F-6574-2014; Gribushin, Andrei/J-4225-2012; Cerrada, Marcos/J-6934-2014; Azzi, Patrizia/H-5404-2012; Calderon, Alicia/K-3658-2014; de la Cruz, Begona/K-7552-2014; Rolandi, Luigi (Gigi)/E-8563-2013; Montanari, Alessandro/J-2420-2012; Raidal, Martti/F-4436-2012; Tomei, Thiago/E-7091-2012; Zalewski, Piotr/H-7335-2013; Tinti, Gemma/I-5886-2013; Ivanov, Andrew/A-7982-2013; Hill, Christopher/B-5371-2012; Liu, Sheng/K-2815-2013; Venturi, Andrea/J-1877-2012; Wimpenny, Stephen/K-8848-2013; Markina, Anastasia/E-3390-2012; Lokhtin, Igor/D-7004-2012; Kadastik, Mario/B-7559-2008; Mundim, Luiz/A-1291-2012; De La Cruz Burelo, Eduard/B-9802-2013; Santaolalla, Javier/C-3094-2013; Alves, Gilvan/C-4007-2013; Tinoco Mendes, Andre David/D-4314-2011; Wulz, Claudia-Elisabeth/H-5657-2011; Fruhwirth, Rudolf/H-2529-2012; de Jesus Damiao, Dilson/G-6218-2012; tosi, mia/J-5777-2012 OI Sznajder, Andre/0000-0001-6998-1108; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Gerbaudo, Davide/0000-0002-4463-0878; TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; Arce, Pedro/0000-0003-3009-0484; Flix, Josep/0000-0003-2688-8047; Della Ricca, Giuseppe/0000-0003-2831-6982; Paganoni, Marco/0000-0003-2461-275X; Gulmez, Erhan/0000-0002-6353-518X; Seixas, Joao/0000-0002-7531-0842; Vilela Pereira, Antonio/0000-0003-3177-4626; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Belyaev, Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279; Konecki, Marcin/0000-0001-9482-4841; Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680; Matorras, Francisco/0000-0003-4295-5668; Ragazzi, Stefano/0000-0001-8219-2074; Scodellaro, Luca/0000-0002-4974-8330; Calvo Alamillo, Enrique/0000-0002-1100-2963; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Marinho, Franciole/0000-0002-7327-0349; Ferguson, Thomas/0000-0001-5822-3731; Benussi, Luigi/0000-0002-2363-8889; Dahms, Torsten/0000-0003-4274-5476; Grandi, Claudio/0000-0001-5998-3070; Lazzizzera, Ignazio/0000-0001-5092-7531; Dogangun, Oktay/0000-0002-1255-2211; Novaes, Sergio/0000-0003-0471-8549; Codispoti, Giuseppe/0000-0003-0217-7021; Cerrada, Marcos/0000-0003-0112-1691; Azzi, Patrizia/0000-0002-3129-828X; Rolandi, Luigi (Gigi)/0000-0002-0635-274X; Montanari, Alessandro/0000-0003-2748-6373; Tomei, Thiago/0000-0002-1809-5226; Ivanov, Andrew/0000-0002-9270-5643; Hill, Christopher/0000-0003-0059-0779; Wimpenny, Stephen/0000-0003-0505-4908; Mundim, Luiz/0000-0001-9964-7805; De La Cruz Burelo, Eduard/0000-0002-7469-6974; Tinoco Mendes, Andre David/0000-0001-5854-7699; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; de Jesus Damiao, Dilson/0000-0002-3769-1680; FU Austrian Federal Ministry of Science and Research; Belgium Fonds de la Recherche Scientifique; Fonds voor Wetenschappelijk Onderzoek; CNPq; CAPES; FAPERJ; FAPESP; Bulgarian Ministry of Education and Science; CERN; Chinese Academy of Sciences; Ministry of Science and Technology; National Natural Science Foundation of China; Colombian Funding Agency (COL-CIENCIAS); Croatian Ministry of Science, Education and Sport; Research Promotion Foundation, Cyprus; Estonian Academy of Sciences; NICPB; Academy of Finland; Finnish Ministry of Education and Culture; Helsinki Institute of Physics; Institut National de Physique Nucleaire et de Physique des Particules / CNRS; Commissariat a l'Energie Atomique et aux Energies Alternatives / CEA, France; Bundesministerium fur Bildung und Forschung; Deutsche Forschungsgemeinschaft; Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; General Secretariat for Research and Technology, Greece; National Scientific Research Foundation; National Office for Research and Technology, Hungary; Department of Atomic Energy; Department of Science and Technology, India; Institute for Studies in Theoretical Physics and Mathematics, Iran; Science Foundation, Ireland; Istituto Nazionale di Fisica Nucleare, Italy; Korean Ministry of Education, Science and Technology; World Class University program of NRF, Korea; Lithuanian Academy of Sciences; CINVESTAV; CONACYT; SEP; UASLP-FAI; Ministry of Science and Innovation, New Zealand; Pakistan Atomic Energy Commission; State Commission for Scientific Research, Poland; Fundacao para a Ciencia e a Tecnologia, Portugal; JINR (Armenia); JINR (Belarus); JINR (Georgia); JINR (Ukraine); JINR (Uzbekistan); Ministry of Science and Technologies of the Russian Federation; Russian Ministry of Atomic Energy; Ministry of Science and Technological Development of Serbia; Ministerio de Ciencia e Innovacion; Programa Consolider-Ingenio, Spain; ETH Board; ETH Zurich; PSI; SNF; UniZH; Canton Zurich; SER; National Science Council, Taipei; Scientific and Technical Research Council of Turkey; Turkish Atomic Energy Authority; Science and Technology Facilities Council, U.K.; US Department of Energy; US National Science Foundation; Marie-Curie programme (European Union); European Research Council (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Associazione per lo Sviluppo Scientifico e Tecnologico del Piemonte (Italy); Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Council of Science and Industrial Research, India FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC machine, and thank the technical and administrative staff sat CERN and other CMS institutes for their contributions. This work was supported by the Austrian Federal Ministry of Science and Research; the Belgium Fonds de la Recherche Scientifique, and Fonds voor Wetenschappelijk Onderzoek; the Brazilian Funding Agencies (CNPq, CAPES, FAPERJ, and FAPESP); the Bulgarian Ministry of Education and Science; CERN; the Chinese Academy of Sciences, Ministry of Science and Technology, and National Natural Science Foundation of China; the Colombian Funding Agency (COL-CIENCIAS); the Croatian Ministry of Science, Education and Sport; the Research Promotion Foundation, Cyprus; the Estonian Academy of Sciences and NICPB; the Academy of Finland, Finnish Ministry of Education and Culture, and Helsinki Institute of Physics; the Institut National de Physique Nucleaire et de Physique des Particules / CNRS, and Commissariat a l'Energie Atomique et aux Energies Alternatives / CEA, France; the Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft, and Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; the General Secretariat for Research and Technology, Greece; the National Scientific Research Foundation, and National Office for Research and Technology, Hungary; the Department of Atomic Energy and the Department of Science and Technology, India; the Institute for Studies in Theoretical Physics and Mathematics, Iran; the Science Foundation, Ireland; the Istituto Nazionale di Fisica Nucleare, Italy; the Korean Ministry of Education, Science and Technology and the World Class University program of NRF, Korea; the Lithuanian Academy of Sciences; the Mexican Funding Agencies (CINVESTAV, CONACYT, SEP, and UASLP-FAI); the Ministry of Science and Innovation, New Zealand; the Pakistan Atomic Energy Commission; the State Commission for Scientific Research, Poland; the Fundacao para a Ciencia e a Tecnologia, Portugal; JINR (Armenia, Belarus, Georgia, Ukraine, Uzbekistan); the Ministry of Science and Technologies of the Russian Federation, and Russian Ministry of Atomic Energy; the Ministry of Science and Technological Development of Serbia; the Ministerio de Ciencia e Innovacion, and Programa Consolider-Ingenio 2010, Spain; the Swiss Funding Agencies (ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER); the National Science Council, Taipei; the Scientific and Technical Research Council of Turkey, and Turkish Atomic Energy Authority; the Science and Technology Facilities Council, U.K.; the US Department of Energy, and the US National Science Foundation.; Individuals have received support from the Marie-Curie programme and the European Research Council (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Associazione per lo Sviluppo Scientifico e Tecnologico del Piemonte (Italy); the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); and the Council of Science and Industrial Research, India. NR 50 TC 12 Z9 12 U1 0 U2 57 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD NOV PY 2012 IS 11 AR 067 DI 10.1007/JHEP11(2012)067 PG 40 WC Physics, Particles & Fields SC Physics GA 052LG UT WOS:000312198500002 ER PT J AU Fleutot, B Miller, JB Gellman, AJ AF Fleutot, Benoit Miller, James B. Gellman, Andrew J. TI Apparatus for deposition of composition spread alloy films: The rotatable shadow mask SO JOURNAL OF VACUUM SCIENCE & TECHNOLOGY A LA English DT Article DE electron beam deposition; masks; metallic thin films ID COMBINATORIAL CHEMISTRY; INORGANIC MATERIALS; MATERIAL LIBRARIES; DRUG DISCOVERY; THIN-FILMS; SURFACES; MO(110); SCIENCE AB Composition spread alloy films (CSAFs) are materials libraries used for high throughput investigations of multicomponent materials such as alloys, A(x)B(y)C(1-x-y). CSAFs are prepared such that the alloy film has a lateral spatial gradient in its local composition; thus, they include a set of alloy samples with a distribution of compositions that spans a continuous region of composition space (x,y). A tool based on the shadow mask concept has been developed for generating composition gradients, but modified to allow rotation of the shadow mask during CSAF deposition. The tool allows deposition of CSAFs containing up to four elements with rotatable shadow masks between each of the four electron beam evaporation sources and the deposition substrate. This allows codeposition of any combination of up to four components. In the case of the ternary A(x)B(y)C(1-x-y) CSAFs, the three components can be deposited such that the resulting CSAF spans the entire ternary alloy composition space (x = 0 -> 1, y = 0 -> 1 - x) and, furthermore, contains all three binary alloys A(x)B(1-x), A(x)C(1-x), and BxC1-x (x = 0 -> 1) and all three pure components. The innovation of the rotatable shadow masks also allows preparation of CSAFs that magnify selected regions of the composition space (x = x(min) -> x(max), y = y(min) -> 1 - x). Herein, we describe the design and performance of this new CSAF deposition tool and assess its merits and limitations with respect to other methods for CSAF preparation. (C) 2012 American Vacuum Society. [http://dx.doi.org/10.1116/1.4766194] C1 [Miller, James B.; Gellman, Andrew J.] US DOE, NETL, RUA, Pittsburgh, PA 15236 USA. [Fleutot, Benoit; Miller, James B.; Gellman, Andrew J.] Carnegie Mellon Univ, Dept Chem Engn, Pittsburgh, PA 15213 USA. RP Gellman, AJ (reprint author), US DOE, NETL, RUA, Pittsburgh, PA 15236 USA. EM gellman@cmu.edu RI Gellman, Andrew/M-2487-2014 OI Gellman, Andrew/0000-0001-6618-7427 FU NSF [CBET-0923083]; RES [DE-FE0004000]; Department of Energy, National Energy Technology Laboratory, an agency of the United States Government through URS Energy & Construction, Inc. FX Transfer Engineering and Manufacturing, Inc. (Fremont, CA) fabricated the RSM-CSAF deposition tool. Support is acknowledged from the NSF under Grant No. CBET-0923083. As part of the National Energy Technology Laboratory's Regional University Alliance (NETL-RUA), a collaborative initiative of the NETL, this technical effort was performed under the RES Contract No. DE-FE0004000. This project was funded, in part, by the Department of Energy, National Energy Technology Laboratory, an agency of the United States Government, through a support contract with URS Energy & Construction, Inc. Neither the United States Government nor any agency thereof, nor any of their employees, nor URS Energy & Construction, Inc., nor any of their employees, makes any warranty, expressed or implied, or assumes any legal liability or responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would not infringe privately owned rights. Reference herein to any specific commercial product, process, or service by trade name, trademark, manufacturer, or otherwise does not necessarily constitute or imply its endorsement, recommendation, or favoring by the United States Government or any agency thereof. The views and opinions of authors expressed herein do not necessarily state or reflect those of the United States Government or any agency thereof. NR 30 TC 8 Z9 8 U1 4 U2 40 PU A V S AMER INST PHYSICS PI MELVILLE PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA SN 0734-2101 J9 J VAC SCI TECHNOL A JI J. Vac. Sci. Technol. A PD NOV PY 2012 VL 30 IS 6 AR 061511 DI 10.1116/1.4766194 PG 10 WC Materials Science, Coatings & Films; Physics, Applied SC Materials Science; Physics GA 042GA UT WOS:000311458500026 ER PT J AU Kerber, P Porter, LM McCullough, LA Kowalewski, T Engelhard, M Baer, D AF Kerber, Pranita Porter, Lisa M. McCullough, Lynne A. Kowalewski, Tomasz Engelhard, Mark Baer, Donald TI Study of surface cleaning methods and pyrolysis temperatures on nanostructured carbon films using x-ray photoelectron spectroscopy SO JOURNAL OF VACUUM SCIENCE & TECHNOLOGY A LA English DT Article DE annealing; carbon; electrical resistivity; graphitisation; nanofabrication; nanostructured materials; polymer blends; polymer films; porosity; pyrolysis; surface composition; X-ray photoelectron spectra ID TRANSFER RADICAL POLYMERIZATION; BLOCK-COPOLYMERS; ACRYLONITRILE AB Nanostructured carbon (ns-C) films fabricated by stabilization and pyrolysis of diblock copolymers are of interest for a variety of electrical/electronic applications due to their chemical inertness, high-temperature insensitivity, very high surface area, and tunable electrical resistivity over a wide range [Kulkarni , Synth. Met. 159, 177 (2009)]. Because of their high porosity and associated high specific surface area, controlled surface cleaning studies are important for fabricating electronic devices from these films. In this study, quantification of surface composition and surface cleaning studies on ns-C films synthesized by carbonization of diblock copolymers of polyacrylonitrile-b-poly(n-butyl acrylate) at two different temperatures were carried out. X-ray photoelectron spectroscopy was used for elemental analysis and to determine the efficacy of various surface cleaning methods for ns-C films and to examine the polymer residues in the films. The in-situ surface cleaning methods included HF vapor treatment, vacuum annealing, and exposure to UV-ozone. Quantitative analysis of high-resolution XPS scans showed 11 at. % nitrogen was present in the films pyrolyzed at 600 degrees C, suggesting incomplete denitrogenation of the copolymer films. The nitrogen atomic concentration decreased significantly for films pyrolyzed at 900 degrees C confirming extensive denitrogenation at that temperature. Furthermore, quantitative analysis of nitrogen subpeaks indicated higher loss of nitrogen atoms residing at the edge of graphitic clusters relative to that of nitrogen atoms within the graphitic clusters, suggesting higher graphitization with increasing pyrolysis temperature. Of the surface cleaning methods investigated, in-situ annealing of the films at 300 degrees C for 40 min was found to be the most efficacious in removing adventitious carbon and oxygen impurities from the surface. (C) 2012 American Vacuum Society. [http://dx.doi.org/10.1116/1.4759238] C1 [Kerber, Pranita; Porter, Lisa M.] Carnegie Mellon Univ, Dept Mat Sci & Engn, Pittsburgh, PA 15213 USA. [McCullough, Lynne A.; Kowalewski, Tomasz] Carnegie Mellon Univ, Dept Chem, Pittsburgh, PA 15213 USA. [Engelhard, Mark; Baer, Donald] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. RP Kerber, P (reprint author), Carnegie Mellon Univ, Dept Mat Sci & Engn, 5000 Forbes Ave, Pittsburgh, PA 15213 USA. EM pranitak@alumni.cmu.edu OI Kowalewski, Tomasz/0000-0002-3544-554X; Engelhard, Mark/0000-0002-5543-0812 FU National Science Foundation [DMR-0304508]; Department of Energy's Office of Biological and Environmental Research FX This research was supported by the National Science Foundation under Award No. DMR-0304508. The XPS portion of this research was performed using EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. The authors acknowledge the help of Dr. C. Tang for the deposition of some PAN-b-PBA polymers using zone-casting techniques and Dr. Rui Zhang for the AFM image. NR 17 TC 1 Z9 1 U1 2 U2 15 PU A V S AMER INST PHYSICS PI MELVILLE PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA SN 0734-2101 EI 1520-8559 J9 J VAC SCI TECHNOL A JI J. Vac. Sci. Technol. A PD NOV PY 2012 VL 30 IS 6 AR 061407 DI 10.1116/1.4759238 PG 6 WC Materials Science, Coatings & Films; Physics, Applied SC Materials Science; Physics GA 042GA UT WOS:000311458500015 ER PT J AU Liu, SS Ma, BH Narayanan, M Tong, S Koritala, R Balachandran, U AF Liu, Shanshan Ma, Beihai Narayanan, Manoj Tong, Sheng Koritala, Rachel Balachandran, Uthamalingam TI Microstructure and electrical properties of LaNiO3 thin films by RF sputtering for the growth of (Pb,La)( Zr,Ti)O-3 films on silicon and nickel substrates SO JOURNAL OF VACUUM SCIENCE & TECHNOLOGY A LA English DT Article DE annealing; buffer layers; crystal microstructure; ferroelectric materials; ferroelectric thin films; lanthanum compounds; lead compounds; nickel; silicon; sputter deposition; texture; X-ray diffraction ID DIELECTRIC-PROPERTIES; METAL FOILS; FERROELECTRIC DEVICES; SOLUTION DEPOSITION; PLZT FILMS; PZT; ELECTRODES; STRESS; TEMPERATURE; FABRICATION AB Conductive LaNiO3 (LNO) thin films were deposited on Si substrates by RF sputtering at room temperature to 600 degrees C. X-ray diffraction of the LNO films showed that preferred orientation varied from (100) below 500 degrees C to (110) at 600 degrees C at deposition temperature of 200-600 degrees C. The room temperature resistivity was 2250-3400 mu Omega-cm at the range of 200 degrees C similar to 500 degrees C. The LNO films, deposited at room temperature, were postannealed in air from 500 to 800 degrees C, and the resistivity value was 280 mu Omega-cm at a postannealing temperature of 600 degrees C. Subsequently, sol-gel derived (Pb,La)(Zr,Ti)O-3 thin films were deposited on LNO-buffered nickel substrates and characterized, the results were compared to those of the same films on silicon substrates. The comparison demonstrated that the performance characteristics of the LNO-buffered nickel foils are similar to those of LNO-buffered silicon substrates. Thus, LNO films prepared by the sputtering method can act as an effective barrier layer on nickel substrates for embedded microelectronic devices. (C) 2012 American Vacuum Society. [http://dx.doi.org/10.1116/1.4752084] C1 [Liu, Shanshan; Ma, Beihai; Narayanan, Manoj; Tong, Sheng; Balachandran, Uthamalingam] Argonne Natl Lab, Div Energy Syst, Argonne, IL 60439 USA. [Koritala, Rachel] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Liu, SS (reprint author), Argonne Natl Lab, Div Energy Syst, 9700 S Cass Ave, Argonne, IL 60439 USA. EM sliu@anl.gov RI Liu, Shanshan/A-6143-2012; Tong, Sheng/A-2129-2011; Ma, Beihai/I-1674-2013 OI Tong, Sheng/0000-0003-0355-7368; Ma, Beihai/0000-0003-3557-2773 FU U.S. Department of Energy, Vehicle Technologies Program [DE-AC02-06CH11357] FX This work was funded by the U.S. Department of Energy, Vehicle Technologies Program, under Contract DE-AC02-06CH11357. This study benefited from use of the Electron Microscopy Center (EMC) at Argonne National Laboratory. NR 42 TC 0 Z9 1 U1 3 U2 25 PU A V S AMER INST PHYSICS PI MELVILLE PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA SN 0734-2101 J9 J VAC SCI TECHNOL A JI J. Vac. Sci. Technol. A PD NOV PY 2012 VL 30 IS 6 AR 061505 DI 10.1116/1.4752084 PG 8 WC Materials Science, Coatings & Films; Physics, Applied SC Materials Science; Physics GA 042GA UT WOS:000311458500020 ER PT J AU Tran, HNN Brechenmacher, L Aldrich, JT Clauss, TR Gritsenko, MA Hixson, KK Libault, M Tanaka, K Yang, F Yao, QM Pasa-Tolic, L Xu, D Nguyen, HT Stacey, G AF Tran Hong Nha Nguyen Brechenmacher, Laurent Aldrich, Joshua T. Clauss, Therese R. Gritsenko, Marina A. Hixson, Kim K. Libault, Marc Tanaka, Kiwamu Yang, Feng Yao, Qiuming Pasa-Tolic, Ljiljana Xu, Dong Nguyen, Henry T. Stacey, Gary TI Quantitative Phosphoproteomic Analysis of Soybean Root Hairs Inoculated with Bradyrhizobium japonicum SO MOLECULAR & CELLULAR PROTEOMICS LA English DT Article ID SYMBIOTIC NODULE DEVELOPMENT; RECEPTOR-LIKE KINASES; ACTIN CYTOSKELETON; RHIZOBIAL INFECTION; MASS-SPECTROMETRY; SIGNAL PEPTIDES; TOBACCO CELLS; POLAR GROWTH; POLLEN TUBES; DATA SETS AB Root hairs are single hair-forming cells on roots that function to increase root surface area, enhancing water and nutrient uptake. In leguminous plants, root hairs also play a critical role as the site of infection by symbiotic nitrogen fixing rhizobia, leading to the formation of a novel organ, the nodule. The initial steps in the rhizobia-root hair infection process are known to involve specific receptor kinases and subsequent kinase cascades. Here, we characterize the phosphoproteome of the root hairs and the corresponding stripped roots (i.e. roots from which root hairs were removed) during rhizobial colonization and infection to gain insight into the molecular mechanism of root hair cell biology. We chose soybean (Glycine max L.), one of the most important crop plants in the legume family, for this study because of its larger root size, which permits isolation of sufficient root hair material for phosphoproteomic analysis. Phosphopeptides derived from root hairs and stripped roots, mock inoculated or inoculated with the soybean-specific rhizobium Bradyrhizobium japonicum, were labeled with the isobaric tag eight-plex iTRAQ, enriched using Ni-NTA magnetic beads and subjected to nanoRPLC-MS/MS1 analysis using HCD and decision tree guided CID/ETD strategy. A total of 1625 unique phosphopeptides, spanning 1659 nonredundant phosphorylation sites, were detected from 1126 soybean phosphoproteins. Among them, 273 phosphopeptides corresponding to 240 phosphoproteins were found to be significantly regulated (>1.5-fold abundance change) in response to inoculation with B. japonicum. The data reveal unique features of the soybean root hair phosphoproteome, including root hair and stripped root-specific phosphorylation suggesting a complex network of kinase-substrate and phosphatase-substrate interactions in response to rhizobial inoculation. Molecular & Cellular Proteomics 11: 10.1074/mcp.M112.018028,1140-1155, 2012. C1 [Tran Hong Nha Nguyen; Brechenmacher, Laurent; Tanaka, Kiwamu; Nguyen, Henry T.; Stacey, Gary] Univ Missouri, Div Plant Sci, CS Bond Life Sci Ctr, Columbia, MO 65211 USA. [Tran Hong Nha Nguyen; Brechenmacher, Laurent; Tanaka, Kiwamu; Nguyen, Henry T.; Stacey, Gary] Univ Missouri, Natl Ctr Soybean Biotechnol, Columbia, MO 65211 USA. [Tran Hong Nha Nguyen] Pacific NW Natl Lab, Vietnam Educ Fdn, Richland, WA 99352 USA. [Aldrich, Joshua T.; Hixson, Kim K.; Pasa-Tolic, Ljiljana] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Clauss, Therese R.; Gritsenko, Marina A.; Yang, Feng] Pacific NW Natl Lab, Fundamental & Computat Sci Div, Richland, WA 99352 USA. [Libault, Marc] Univ Oklahoma, Dept Bot & Microbiol, Norman, OK 73019 USA. [Yao, Qiuming; Xu, Dong] Univ Missouri, CS Bond Life Sci Ctr, Dept Comp Sci, Columbia, MO 65211 USA. [Stacey, Gary] Univ Missouri, Div Biochem, Christopher S Bond Life Sci Ctr 271E, Columbia, MO 65211 USA. RP Stacey, G (reprint author), Univ Missouri, Div Plant Sci, Christopher S Bond Life Sci Ctr 271E, Columbia, MO 65211 USA. EM staceyg@missouri.edu RI Tanaka, Kiwamu/E-9942-2013 OI Tanaka, Kiwamu/0000-0001-5045-560X FU National Science Foundation [DBI-0421620]; United Soybean Board; US Department of Energy (DOE) Office of Biological and Environmental Research; NIH National Center for Research Resources [RR018522]; DOE [DE-AC05-76RLO 1830] FX This work was supported by the Plant Genome Program (DBI-0421620) from the National Science Foundation (to GS, LP-T, DX) and by funding from the United Soybean Board (to HN, GS, DX).; The authors acknowledge that portions of this work were supported by the US Department of Energy (DOE) Office of Biological and Environmental Research and by the NIH National Center for Research Resources (RR018522). Work was performed in the Environmental Molecular Science Laboratory (EMSL), a DOE national scientific user facility located on the campus of Pacific Northwest National Laboratory (PNNL) in Richland, Washington. PNNL is a multi-program national laboratory operated by Battelle for the DOE under contract DE-AC05-76RLO 1830. NR 69 TC 51 Z9 53 U1 5 U2 55 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 1535-9476 J9 MOL CELL PROTEOMICS JI Mol. Cell. Proteomics PD NOV PY 2012 VL 11 IS 11 BP 1140 EP 1155 DI 10.1074/mcp.M112.018028 PG 16 WC Biochemical Research Methods SC Biochemistry & Molecular Biology GA 067EP UT WOS:000313277100004 ER PT J AU van Duijn, E Barbu, IM Barendreg, A Jore, MM Wiedenheft, B Lundgren, M Westra, ER Brouns, SJJ Doudna, JA van der Oost, J Heck, AJR AF van Duijn, Esther Barbu, Ioana M. Barendreg, Arjan Jore, Matthijs M. Wiedenheft, Blake Lundgren, Magnus Westra, Edze R. Brouns, Stan J. J. Doudna, Jennifer A. van der Oost, John Heck, Albert J. R. TI Native Tandem and Ion Mobility Mass Spectrometry Highlight Structural and Modular Similarities in Clustered-Regularly-Interspaced Shot-Palindromic-Repeats (CRISPR)-associated Protein Complexes From Escherichia coli and Pseudomonas aeruginosa SO MOLECULAR & CELLULAR PROTEOMICS LA English DT Article ID BACTERIAL IMMUNE-SYSTEM; CRISPR-CAS SYSTEMS; GAS-PHASE; SUBUNIT ARCHITECTURE; ANTIVIRAL DEFENSE; SMALL RNA; DNA; RECOGNITION; PROKARYOTES; SEQUENCE AB The CRISPR/Cas (clustered regularly interspaced short palindromic repeats/CRISPR-associated genes) immune system of bacteria and archaea provides acquired resistance against viruses and plasmids, by a strategy analogous to RNA-interference. Key components of the defense system are ribonucleoprotein complexes, the composition of which appears highly variable in different CRISPR/Cas subtypes. Previous studies combined mass spectrometry, electron microscopy, and small angle x-ray scattering to demonstrate that the E. coli Cascade complex (405 kDa) and the P. aeruginosa Csy-complex (350 kDa) are similar in that they share a central spiral-shaped hexameric structure, flanked by associating proteins and one CRISPR RNA. Recently, a cryo-electron microscopy structure of Cascade revealed that the CRISPR RNA molecule resides in a groove of the hexameric backbone. For both complexes we here describe the use of native mass spectrometry in combination with ion mobility mass spectrometry to assign a stable core surrounded by more loosely associated modules. Via computational modeling subcomplex structures were proposed that relate to the experimental IMMS data. Despite the absence of obvious sequence homology between several subunits, detailed analysis of sub-complexes strongly suggests analogy between subunits of the two complexes. Probing the specific association of E. coli Cascade/crRNA to its complementary DNA target reveals a conformational change. All together these findings provide relevant new information about the potential assembly process of the two CRISPR-associated complexes. Molecular & Cellular Proteomics 11: 10.1074/mcp.M112.020263, 1430-1441, 2012. C1 [van Duijn, Esther; Barbu, Ioana M.; Barendreg, Arjan; Heck, Albert J. R.] Univ Utrecht, Bijvoet Ctr Biomol Res, Biomol Mass Spectrometry & Prote Grp, NL-3584 CH Utrecht, Netherlands. [van Duijn, Esther; Barbu, Ioana M.; Barendreg, Arjan; Heck, Albert J. R.] Univ Utrecht, Utrecht Inst Pharmaceut Sci, NL-3584 CH Utrecht, Netherlands. [van Duijn, Esther; Barbu, Ioana M.; Barendreg, Arjan; Heck, Albert J. R.] Netherlands Prote Ctr, NL-3584 CH Utrecht, Netherlands. [Jore, Matthijs M.; Lundgren, Magnus; Westra, Edze R.; Brouns, Stan J. J.; van der Oost, John] Wageningen Univ, Microbiol Lab, NL-6703 HB Wageningen, Netherlands. [Wiedenheft, Blake; Doudna, Jennifer A.] Howard Hughes Med Inst, Chevy Chase, MD 20815 USA. [Wiedenheft, Blake; Doudna, Jennifer A.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Lundgren, Magnus] Uppsala Univ, Dept Cell & Mol Biol, S-75123 Uppsala, Sweden. [Doudna, Jennifer A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Doudna, Jennifer A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP van Duijn, E (reprint author), Univ Utrecht, Bijvoet Ctr Biomol Res, Biomol Mass Spectrometry & Prote Grp, Padualaan 8, NL-3584 CH Utrecht, Netherlands. EM e.vanduijn1@uu.nl RI Heck, Albert/D-7098-2011 OI Heck, Albert/0000-0002-2405-4404 FU Netherlands Organization for Scientific Research (NWO) [VENI 700.58.402, VENI 863.08.014]; The Netherlands Proteomics Centre FX This work was supported by the Netherlands Organization for Scientific Research (NWO) (VENI 700.58.402) to E.v.D., and (VENI 863.08.014) to S.J.J.B. We thank The Netherlands Proteomics Centre for financial support. NR 47 TC 36 Z9 36 U1 4 U2 32 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 1535-9476 EI 1535-9484 J9 MOL CELL PROTEOMICS JI Mol. Cell. Proteomics PD NOV PY 2012 VL 11 IS 11 BP 1430 EP 1441 DI 10.1074/mcp.M112.020263 PG 12 WC Biochemical Research Methods SC Biochemistry & Molecular Biology GA 067EP UT WOS:000313277100025 PM 22918228 ER PT J AU Premrov, A Coxon, CE Hackett, R Kirwan, L Richards, KG AF Premrov, Alina Coxon, Catherine E. Hackett, Richard Kirwan, Laura Richards, Karl G. TI Effects of over-winter green cover on groundwater nitrate and dissolved organic carbon concentrations beneath tillage land SO SCIENCE OF THE TOTAL ENVIRONMENT LA English DT Article DE Groundwater; Nitrate; Dissolved organic carbon; Over-winter green cover; Tillage ID SOIL-MOISTURE CONDITIONS; LEACHING LOSSES; CATCH CROPS; MATTER; IRELAND; MANAGEMENT; NITROGEN; GROWTH; DENITRIFICATION; GRASSLANDS AB Application of over-winter green cover (e.g. cover crops) as a measure for reducing nitrate losses from tillage land has been frequently investigated, especially in the unsaturated zone. Monitoring of groundwater is less common in these studies. Studies on groundwater responses to different land treatments can be challenging because they can be influenced by various conditions, such as recharge, seasonal variations, and aquifer properties, often occurring at different time scales than surface water processes. The aim of this study was to evaluate groundwater nitrate (NO3- - N) and dissolved organic carbon (DOC) concentration responses to different over-winter green covers: mustard, natural regeneration and no cover. A field experiment was designed and run for three years on tillage land underlain by a vulnerable sand and gravel aquifer in the south-east of Ireland. Results showed that over-winter green cover growth on tillage land can be an effective measure to reduce groundwater NO3- - N concentrations. A significant decrease in groundwater NO3- - N concentrations was observed under the mustard cover compared to no cover. All treatments, including no cover, showed a decline in groundwater NO3- - N concentrations overtime. A significant increase in groundwater DOC was also observed under the mustard cover. Although the overall groundwater DOC concentrations were low, the increased DOC occurrence in groundwater should be accounted for in carbon balances and could potentially enhance groundwater denitrification in cases where aquifer conditions may favour it. (C) 2012 Elsevier B.V. All rights reserved. C1 [Premrov, Alina; Coxon, Catherine E.] Univ Dublin Trinity Coll, Dept Geol, Sch Nat Sci, Dublin 2, Ireland. [Premrov, Alina; Kirwan, Laura; Richards, Karl G.] TEAGASC, Johnstown Castle Environm Res Ctr, Wexford, Ireland. [Hackett, Richard] TEAGASC, Oak Pk Res Ctr, Carlow, Ireland. [Kirwan, Laura] Waterford Inst Technol, Waterford, Ireland. RP Premrov, A (reprint author), Univ Dublin Trinity Coll, Dept Geol, Sch Nat Sci, Dublin 2, Ireland. EM premrova@tcd.ie; cecoxon@tcd.ie; karl.richards@teagasc.ie RI Richards, Karl/A-5606-2010; Coxon, Catherine/O-7368-2014 OI Richards, Karl/0000-0002-3703-3450; Coxon, Catherine/0000-0002-2911-9115 FU Teagasc Walsh Fellowship; Trinity College Dublin (TCD) FX The authors are grateful for funding provided by the Teagasc Walsh Fellowship and Trinity College Dublin (TCD). Special thanks go to Teagasc, Johnstown Castle, Wexford staff: D. Brennan for laboratory-support, P. Sills, J. Murphy and J. Hogan for field-work help. Special thanks also go to Dr. N. Allott and Dr. C. Rocha (TCD), and to Dr. T. Dittmar and IG.N.A. Suryaputra (MPI-Bremen) for their advice on the Fluorescence Spectrophotometrical analysis. The authors are grateful to Met Eireann, The Irish Meteorological Service, for the provision of meteorological data. NR 65 TC 10 Z9 10 U1 4 U2 36 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0048-9697 J9 SCI TOTAL ENVIRON JI Sci. Total Environ. PD NOV 1 PY 2012 VL 438 BP 144 EP 153 DI 10.1016/j.scitotenv.2012.08.043 PG 10 WC Environmental Sciences SC Environmental Sciences & Ecology GA 065NN UT WOS:000313155300019 PM 22982940 ER PT J AU Solomon, D Lehmann, J Wang, J Kinyangi, J Heymann, K Lu, YS Wirick, S Jacobsen, C AF Solomon, Dawit Lehmann, Johannes Wang, Jian Kinyangi, James Heymann, Karen Lu, Yingshen Wirick, Sue Jacobsen, Chris TI Micro- and nano-environments of C sequestration in soil: A multi-elemental STXM-NEXAFS assessment of black C and organomineral associations SO SCIENCE OF THE TOTAL ENVIRONMENT LA English DT Article DE Biotic exclusion zone; C sequestration; Global C cycling; Organomineral interactions; Spatial inaccessibility; Soft X-ray spectromicroscopy ID X-RAY SPECTROMICROSCOPY; NEAR-EDGE STRUCTURE; INNERSHELL ABSORPTION-SPECTROSCOPY; AL K-EDGE; ORGANIC-MATTER; XANES SPECTROSCOPY; AMINO-ACIDS; CARBONACEOUS MATERIALS; MOLECULAR-STRUCTURE; MARINE PARTICULATE AB Black C is an essential component of the terrestrial C pool and its formation is often credited as a CO2 sink by transferring the fast-cycling C from the atmosphere-biosphere system into slower cycling C in the geosphere. This study is the first multi-element K- (C, N, Ca, Fe, Al and Si) soft-X-ray STXM-NEXAFS investigation conducted at a submicron-scale spatial resolution specifically targeting black C and its interaction with the mineral and non-black C organic matter in the organomineral assemblage. The STXM-NEXAFS micrographs and spectra demonstrated that pyrogenic C was dominated by quinoide, aromatic, phenol, ketone, alcohol, carboxylic and hydroxylated- and ether-linked C species. There was also evidence for the presence of pyridinic, pyridonic, pyrrolic, amine and nitril N functionalities. The non-black C organic matter contained amino acids, amino sugars, nucleic acids and polysaccharides known to exhibit negatively charged carboxylic, phenolic, enolic, thiolate and phosphate functionalities highly reactive towards metal ions and black C. The metal-rich mineral matrix was composed of phyllosilicate clay minerals, Fe and Al hydroxypolycations, oxides, hydroxides and oxyhydroxide that can attract and bind organic biopolymers. STXM-NEXAFS provided evidence for interactive association between pyrogenic C. non-black C organic matter and the mineral oxide and oxyhydroxide communities in the organomineral interface. These intimate associations occurred through a "two-way" direct linkage between black C and the mineral or non-black C organic matter or via a "three-way" indirect association where non-black C organic matter could serve as a molecular cross-linking agent binding black C with the mineral matrix or vice versa where inorganic oxides, hydroxides and polycations could act as a bridge to bind black C with non-black C organic matter. The binding and sequestration of black C in the investigated micro- and nano-C repository environments seem to be the combined action of physical entrapment in seemingly terminal biotic exclusion zone through the action of metal oxides and organic matter induced microaggregation and through molecular-level association ranging from ligand exchange, polyvalent cation bridging to weak hydrophobic interactions including van der Waals and H-bonding. (C) 2012 Elsevier B.V. All rights reserved. C1 [Solomon, Dawit; Lehmann, Johannes; Kinyangi, James; Heymann, Karen] Cornell Univ, Ithaca, NY 14853 USA. [Wang, Jian; Lu, Yingshen] Canadian Light Source Inc, Saskatoon, SK S7N 0X4, Canada. [Wirick, Sue] Natl Synchrotron Light Source, Upton, NY 11973 USA. [Jacobsen, Chris] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Solomon, D (reprint author), Cornell Univ, Ithaca, NY 14853 USA. EM ds278@cornell.edu RI Wang, Jian/M-1805-2013; Jacobsen, Chris/E-2827-2015; Lehmann, Johannes/H-2682-2014 OI Jacobsen, Chris/0000-0001-8562-0353; Lehmann, Johannes/0000-0002-4701-2936 FU Agriculture and Food Research Initiative Competitive Grant of the National Institute of Food and Agriculture (NIFA) [2008-35107-04511]; Geobiology and Low-Temperature Geochemistry Program of the National Science Foundation (NSF) [EAR-0819689] FX This study was supported by grants from the Agriculture and Food Research Initiative Competitive Grant of the National Institute of Food and Agriculture (NIFA) (2008-35107-04511) and the Geobiology and Low-Temperature Geochemistry Program of the National Science Foundation (NSF) (EAR-0819689). The opinions and findings expressed in this material are those of the authors and do not reflect the views of NIFA or NSF. The C K-edge NEXAFS was recorded at X1A1 beamline of the National Synchrotron Light Source (NSLS). The N, Al, Si K-edge, and Ca and Fe L-edge NEXAFS were performed at SM 10ID-1 beamline of the Canadian Light Source (CLS). NR 97 TC 17 Z9 17 U1 7 U2 110 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0048-9697 J9 SCI TOTAL ENVIRON JI Sci. Total Environ. PD NOV 1 PY 2012 VL 438 BP 372 EP 388 DI 10.1016/j.scitotenv.2012.08.071 PG 17 WC Environmental Sciences SC Environmental Sciences & Ecology GA 065NN UT WOS:000313155300044 PM 23022722 ER PT J AU Kushima, A Huang, JY Li, J AF Kushima, Akihiro Huang, Jian Yu Li, Ju TI Quantitative Fracture Strength and Plasticity Measurements of Lithiated Silicon Nanowires by In Situ TEM Tensile Experiments SO ACS NANO LA English DT Article DE constitutive law; battery cyclability; bending; apparent strain vs true strain; ideal strength ID LITHIUM BATTERY ANODES; CORE-SHELL NANOWIRES; HIGH-CAPACITY; ION BATTERIES; SIMULATIONS; ELECTRODES AB We report in situ tensile strength measurement of fully lithiated Si (Li-Si alloy) nanowires inside a transmission electron microscope. A specially designed dual probe with an atomic force microscopy cantilever and a scanning tunneling microscopy electrode was used to conduct lithiation of Si nanowires and then perform in situ tension of the lithiated nanowires. The axial tensile strength decreased from the initial value of 3.6 GPa for the pristine unlithiated Si nanowires to 0.72 GPa for the lithiated Li-Si alloy. We observed large fracture strain ranging from 8% to 16% for Li-Si alloy, 70% of which remained permanent after fracture. This indicates a certain degree of tensile plasticity in the lithiated silicon before fracture, Important for constitutive modeling of the lithium-ion battery cyclability. We also compare the ab initio computed ideal strengths with our measured strengths and attribute the differences to the morphology and flaws in the lithiated nanowires. C1 [Huang, Jian Yu] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA. [Kushima, Akihiro; Li, Ju] MIT, Dept Nucl Sci & Engn, Cambridge, MA 02139 USA. [Kushima, Akihiro; Li, Ju] MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA. RP Huang, JY (reprint author), Sandia Natl Labs, Ctr Integrated Nanotechnol, POB 5800, Albuquerque, NM 87185 USA. EM jhuang@sandia.gov; liju@mit.edu RI Li, Ju/A-2993-2008; Kushima, Akihiro/H-2347-2011 OI Li, Ju/0000-0002-7841-8058; FU Honda Research Institute; NSF [DMR-1008104, DMR-1120901]; AFOSR [FA9550-08-1-0325]; Laboratory Directed Research and Development (LDRD) project at Sandia National Laboratories; Nanostructures for Electrical Energy Storage (NEES), an Energy Frontier Research Center; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DESC0001160]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX A.K. and J.L. acknowledge support by Honda Research Institute, NSF DMR-1008104, DMR-1120901, and AFOSR FA9550-08-1-0325. Portions of this work were supported by a Laboratory Directed Research and Development (LDRD) project at Sandia National Laboratories and partly by Nanostructures for Electrical Energy Storage (NEES), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Award No. DESC0001160. The LDRD supported the development and fabrication of platforms. The NEES center supported the development of TEM techniques. The Sandia-Los Alamos Center for Integrated Nanotechnologies supported the TEM capability. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Company, for the U.S. Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL85000. NR 33 TC 41 Z9 42 U1 10 U2 145 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 EI 1936-086X J9 ACS NANO JI ACS Nano PD NOV PY 2012 VL 6 IS 11 BP 9425 EP 9432 DI 10.1021/nn3037623 PG 8 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 043CY UT WOS:000311521700010 PM 23025575 ER PT J AU Sandberg, RL Padilha, LA Qazilbash, MM Bae, WK Schaller, RD Pietryga, JM Stevens, MJ Baek, B Nam, SW Klimov, VI AF Sandberg, Richard L. Padilha, Lazaro A. Qazilbash, Muhammad M. Bae, Wan Ki Schaller, Richard D. Pietryga, Jeffrey M. Stevens, Martin J. Baek, Burm Nam, Sae Woo Klimov, Victor I. TI Multiexciton Dynamics in Infrared-Emitting Colloidal Nanostructures Probed by a Superconducting Nanowire Single-Photon Detector SO ACS NANO LA English DT Article DE nanocrystal quantum dot; nanorod; carrier multiplication; multiexciton; Auger recombination; superconducting nanowire single-photon detector; photoluminesence ID MULTIPLE EXCITON GENERATION; CARRIER MULTIPLICATION YIELDS; NANOCRYSTAL QUANTUM DOTS; SEMICONDUCTOR NANOCRYSTALS; PBSE; EFFICIENCY; EMISSION; NANORODS AB Carrier multiplication (CM) is the process in Which absorption of a single photon produces multiple electron-hole pairs. Here, we evaluate the effect of particle shape on CM efficiency by conducting a, comparative study of spherical nanocrystal quantum dots (NQDs) and elongated nanorods (NRs) of PbSe using a time-resolved technique that Is based on photon counting in the infrared using a superconducting nanowire single-photon photodetector (SNSPD). Due to its high sensitivity and low noise levels, this technique allows for accurate determination of CM yields, even with the small excitation intensities required for quantitative measurements, and the fairly low emission quantum yields of elongated NR samples. Our measurements indicate an up to similar to 60% Increase in multiexciton yields in NRs versus NQDs which is attributed primarily to a decrease in the electron-hole pair creation energy. These findings suggest that shape control is a promising approach for enhancing the CM process. Further; our. work demonstrates the effectiveness of the SNSPD technique for the rapid screening of CM performance in infrared nanomaterials. C1 [Sandberg, Richard L.; Padilha, Lazaro A.; Qazilbash, Muhammad M.; Bae, Wan Ki; Schaller, Richard D.; Pietryga, Jeffrey M.; Klimov, Victor I.] Los Alamos Natl Lab, Ctr Adv Solar Photophys, Los Alamos, NM 87545 USA. [Schaller, Richard D.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Stevens, Martin J.; Baek, Burm; Nam, Sae Woo] NIST, Boulder, CO 80305 USA. RP Klimov, VI (reprint author), Los Alamos Natl Lab, Ctr Adv Solar Photophys, POB 1663, Los Alamos, NM 87545 USA. EM kilmov@lanl.gov RI Padilha, Lazaro/G-1523-2013; OI Sandberg, Richard/0000-0001-9719-8188; Klimov, Victor/0000-0003-1158-3179 FU U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES); Los Alamos National Laboratory FX This work was performed within the Center for Advanced Solar Photophysics (CASP), an Energy Frontier Research Center funded by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES). We thank E. Dauler, K. Berggren, and J. Stern for providing the SNSPD devices. We thank M. Rabin, M. Croce, and N. Weiss-Burnstein of Los Alamos National Laboratory for help In setting up and maintaining the SNSPD. R.L.S. and M.M.Q. were CASP members funded through Director's Postdoctoral Fellowship at Los Alamos National Laboratory. NR 51 TC 28 Z9 28 U1 1 U2 65 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 J9 ACS NANO JI ACS Nano PD NOV PY 2012 VL 6 IS 11 BP 9532 EP 9540 DI 10.1021/nn3043226 PG 9 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 043CY UT WOS:000311521700021 PM 23020520 ER PT J AU Liang, XG Wi, SJ AF Liang, Xiaogan Wi, Sungjin TI Transport Characteristics of Multichannel Transistors Made from Densely Aligned Sub-10 nm Half-Pitch Graphene Nanoribbons SO ACS NANO LA English DT Article DE nanofabrication; graphene; transistors; block-copolymers; nanoimprint ID LINE-EDGE ROUGHNESS; BLOCK-COPOLYMER; NANOIMPRINT LITHOGRAPHY; FABRICATION; IMPRINT; ARRAYS AB Densely aligned sub 10 nm graphene nanoribbons are desirable for scale-up applications in nanoelectronics. We implemented directed self-assembly of block-copolymers in combination with nanoimprint lithography to pattern sub-10 nm half-pitch nanoribbons over large areas. These graphene nanoribbons have the highest density and uniformity to date. Multichannel field-effect transistors were made from such nanoribbons, and the transport characteristics of transistors were studied. Our work indicates that a large ribbon-to-ribbon width variation in a multichannel FET can lead to nonsynchronized switching characters of multiple graphene channels and thus a poor ON/OFF current ratio. Through process optimization, we have created 8 nm half pitch graphene nanoribbons, with the minimal ribbon-to-ribbon width variation of similar to 2.4 nm (3 sigma value). The corresponding transistors exhibit an ON/OFF current ratio > 10, which is among the highest values ever reported for. transistors consisting of densely arranged graphene nanoribbons. This work provides important insights for optimizing the uniformity and transport properties of lithographically patterned graphene nanostructures. In addition, the presented fabrication route could be further developed for the scalable nanomanufacturing of graphene-based nanoelectronic devices over large areas. C1 [Liang, Xiaogan; Wi, Sungjin] Univ Michigan, Dept Mech Engn, Ann Arbor, MI 48109 USA. [Liang, Xiaogan] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. RP Liang, XG (reprint author), Univ Michigan, Dept Mech Engn, Ann Arbor, MI 48109 USA. EM xiaoganl@umich.edu FU Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U.S. Department of Energy [DE-AC02-05CH11231]; Department of Mechanical Engineering, University of Michigan; NSF [DMR-0320740] FX The early stage nanofabrication test was partially supported by the Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The optimization of the nanofabrication process and the device characterization were finished at the NanoEngineering and NanoDevice Laboratory, University of Michigan (UM), which were supported by the new faculty start-up fund from the Department of Mechanical Engineering, University of Michigan. The authors would like to thank Dr. D. Olynick, Dr. S. Cabrini, and Prof. J. Bokor for the helpful discussion during the early concept test at the Molecular Foundry, Lawrence Berkeley National Laboratory; Prof. A. Boehman for his precious advice in revising the manuscript; staffs of the University of Michigan's North Campus Electron Microbeam Analysis Laboratory and NSF Grant No. DMR-0320740 for providing the support of SEM Imaging. NR 33 TC 44 Z9 44 U1 7 U2 78 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 EI 1936-086X J9 ACS NANO JI ACS Nano PD NOV PY 2012 VL 6 IS 11 BP 9700 EP 9710 DI 10.1021/nn303127y PG 11 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 043CY UT WOS:000311521700039 PM 23078122 ER PT J AU Zhou, YG Wang, ZG Yang, P Zu, XT Yang, L Sun, X Gao, F AF Zhou, Yungang Wang, Zhiguo Yang, Ping Zu, Xiaotao Yang, Li Sun, Xin Gao, Fei TI Tensile Strain Switched Ferromagnetism in Layered NbS2 and NbSe2 SO ACS NANO LA English DT Article DE NbS2; NbSe2; biaxial strain; magnetism; density functional theory ID MAGNETIC-PROPERTIES; GRAPHENE; MOS2; TRANSISTORS; MONOLAYER; NANOCOMPOSITE; EXFOLIATION; NANOSHEETS; TRANSPORT AB Developing approaches to effectively induce and control the magnetic states, is critical to the use of magnetic nanostructures in quantum-information devices but is still challenging. Here we have demonstrated, by employing the density functional theory calculations, the existence of infinite magnetic sheets with structural integrity and magnetic homogeneity. Examination of a series of transition metal dichalcogenides shows that the biaxial tensile strained NbS2 and NbSe2 structures can be magnetized with a ferromagnetic character due to the competitive effects of through-bond interaction and through-space interaction. The estimated Curie temperatures (387 and 542 K under the 10% strain for NbS2 and NbSe2 structures, respectively) suggest that the unique ferromagnetic character can be achieved above room temperature. The self-exchange of population between 4d orbitals of the Nb atom that leads to exchange splitting is the mechanism behind the transition of the spin moment. The induced magnetic Moments can be significantly enhanced by the tensile strain, even giving rise to a half metallic character with a strong spin polarization around, the Fermi level, Given the recent progress in achieving the desired strain on two-dimensional nanostructures, such as graphene and a BN layer, in a controlled way, we believe that our calculated results are suitable for experimental verification and implementation, opening a new path to explore the spintronics in pristine-two-dimensional nanostructures. C1 [Zhou, Yungang; Wang, Zhiguo; Zu, Xiaotao; Yang, Li] Univ Elect Sci & Technol China, Dept Appl Phys, Chengdu 610054, Peoples R China. [Zhou, Yungang; Yang, Ping; Sun, Xin; Gao, Fei] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Zu, XT (reprint author), Univ Elect Sci & Technol China, Dept Appl Phys, Chengdu 610054, Peoples R China. EM xtzu@uestc.edu.cn; fei.gao@pnnl.gov RI Wang, Zhiguo/B-7132-2009; OI Yang, Ping/0000-0003-4726-2860 FU Division of Materials Sciences and Engineering, Office of Basic Energy Sciences, U.S. Department of Energy [DE-AC05-76RL01830]; National Natural Science Foundation of China [61178018] FX This study was financially supported by the Division of Materials Sciences and Engineering, Office of Basic Energy Sciences, U.S. Department of Energy, under Contract DE-AC05-76RL01830. The authors also wish to thank the Molecular Science Computing Facility in the Environmental Molecular Sciences Laboratory at the Pacific Northwest National Laboratory for a grant of computer time. This study was also supported financially by the National Natural Science Foundation of China (61178018). NR 65 TC 86 Z9 87 U1 32 U2 379 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 EI 1936-086X J9 ACS NANO JI ACS Nano PD NOV PY 2012 VL 6 IS 11 BP 9727 EP 9736 DI 10.1021/nn303198w PG 10 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 043CY UT WOS:000311521700042 PM 23057936 ER PT J AU Lukashev, PV Paudel, TR Lopez-Encarnacion, JM Adenwalla, S Tsymbal, EY Velev, JP AF Lukashev, Pavel V. Paudel, Tula R. Lopez-Encarnacion, Juan M. Adenwalla, Shireen Tsymbal, Evgeny Y. Velev, Julian P. TI Ferroelectric Control of Magnetocrystalline Anisotropy at Cobalt/Poly(vinylidene fluoride) Interfaces SO ACS NANO LA English DT Article DE electric control of magnetization; magnetoelectric effect; magnetocrystalline anisotropy; ferromagnet/ferroelectric interface; organic ferroelectric ID MAGNETIC TUNNEL-JUNCTIONS; MAGNETOELECTRIC MATERIALS; ATOMIC LAYERS; FERROMAGNETS; IRON AB Electric field control of magnetization is one of the promising avenues for achieving high-density energy-efficient magnetic data storage. Ferroelectric materials can be especially useful for that purpose as a source of very large switchable electric fields when interfaced with a ferromagnet. Organic ferroelectrics, such as poly(vinylidene fluoride) (PVDF), have an additional advantage of being weakly bonded to the ferromagnet, thus minimizing undesirable effects such as interface chemical modification and/or strain coupling. In this work we use first-principles density functional calculations of Co/PVDF heterostructures to demonstrate the effect of ferroelectric polarization of PVDF on the interface magnetocrystalline anisotropy that controls the magnetization orientation. We show that switching of the polarization direction alters the magnetocrystalline anisotropy energy of the adjacent Co layer by about 50%, driven by the modification of the screening charge induced by ferroelectric polarization. The effect is reduced with Co oxidation at the interface due to quenching the Interface magnetization. Our results provide a new insight into the mechanism of the magnetoelectric coupling at organic ferroelectric/ferromagnet Interfaces and suggest ways to achieve the desired functionality in practice. C1 [Lukashev, Pavel V.; Paudel, Tula R.; Adenwalla, Shireen; Tsymbal, Evgeny Y.; Velev, Julian P.] Univ Nebraska, Dept Phys & Astron, Lincoln, NE 68588 USA. [Lukashev, Pavel V.; Paudel, Tula R.; Adenwalla, Shireen; Tsymbal, Evgeny Y.; Velev, Julian P.] Univ Nebraska, Nebraska Ctr Mat & Nanosci, Lincoln, NE 68588 USA. [Lopez-Encarnacion, Juan M.; Velev, Julian P.] Univ Puerto Rico, Dept Phys, San Juan, PR 00931 USA. [Lopez-Encarnacion, Juan M.; Velev, Julian P.] Univ Puerto Rico, Inst Funct Nanomat, San Juan, PR 00931 USA. [Lopez-Encarnacion, Juan M.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60349 USA. RP Tsymbal, EY (reprint author), Univ Nebraska, Dept Phys & Astron, Lincoln, NE 68588 USA. EM tsymbal@unl.edu; Jvelev@gmail.com RI Tsymbal, Evgeny/G-3493-2013 FU NSF MRSEC [DMR-0906443]; NSF EPSCoR [EPS-1010674]; NSF [EPS-1010094, EPS-1002410, DMR-1105474] FX This work was supported at the University of Nebraska-Lincoln (UNL) by NSF MRSEC (Grant No. DMR-0906443) and NSF EPSCoR (Grant No. EPS-1010674) and at the University of Puerto Rico by NSF (Grants Nos. EPS-1010094, EPS-1002410, and DMR-1105474). Computations were performed at the Holland Computing Center at UNL and Center for Nanophase Materials Sciences at Oak Ridge National Laboratory. NR 47 TC 22 Z9 22 U1 6 U2 104 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 EI 1936-086X J9 ACS NANO JI ACS Nano PD NOV PY 2012 VL 6 IS 11 BP 9745 EP 9750 DI 10.1021/nn303212h PG 6 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 043CY UT WOS:000311521700044 PM 23039083 ER PT J AU Wu, G Mack, NH Gao, W Ma, SG Zhong, RQ Han, JT Baldwin, JK Zelenay, P AF Wu, Gang Mack, Nathan H. Gao, Wei Ma, Shuguo Zhong, Ruiqin Han, Jiantao Baldwin, Jon K. Zelenay, Piotr TI Nitrogen Doped Graphene-Rich Catalysts Derived from Heteroatom Polymers for Oxygen Reduction in Nonaqueous Lithium-O-2 Battery Cathodes SO ACS NANO LA English DT Article DE graphene; nitrogen doping; heteroatom polymer; non-precious-metal catalysts; oxygen reduction; Li-O-2 battery ID RECHARGEABLE LI-O-2 BATTERIES; PEM FUEL-CELLS; AIR BATTERIES; METAL CATALYSTS; GRAPHITE OXIDE; ELECTROCATALYTIC ACTIVITY; CARBON; POLYANILINE; IRON; SUPERCAPACITORS AB In this work, we present a synthesis approach for nitrogen-doped graphene-Sheet-like nanostructures via the graphitization of a heteroatom polymer, in particular, polyaniline, under the catalysis of a cobalt species using multiwalled carbon nanotubes (MWNTs) as a supporting template. The graphene-rich composite catalysts (Co-N-MWNTs) exhibit substantially improved activity for oxygen reduction in nonaqueous lithium-Ion electrolyte as compared to those of currently used carbon blacks and Pt/carbon catalysts, evidenced by both rotating disk electrode and Li-O-2 battery experiments. The synthesis-structure-activity correlations for the graphene nanostructures were explored by tuning their synthetic chemistry (support, nitrogen precursor, heating temperature, and transition metal type and content) to investigate how the resulting morphology and nitrogen-doping functionalities (e.g., pyridinic, pyrrolic, and quaternary) influence the catalyst activity. In particular, an optimal. temperature for heat treatment during synthesis is critical to creating a high-surface-area catalyst with favorable nitrogen doping. The sole Co phase, Co9S8, was present In the catalyst but plays a negligible role in 'ORR. Nevertheless; the addition of Co species in the synthesis is indispensable for achieving high activity, due to its effects on the final catalyst morphology and structure, Including surface area, nitrogen doping, and graphene formation. This new route for the preparation of a nitrogen-doped graphene nanocomposite with carbon nanotube offers synthetic control of morphology and. nitrogen functionality and shows promise for applications in nonaqueous oxygen reduction electrocatalysis for Li-O-2 battery cathodes. C1 [Wu, Gang; Gao, Wei; Zhong, Ruiqin; Han, Jiantao; Baldwin, Jon K.; Zelenay, Piotr] Los Alamos Natl Lab, Mat Phys & Applicat Div, Los Alamos, NM 87545 USA. [Mack, Nathan H.] Los Alamos Natl Lab, Div Chem, Los Alamos, NM 87545 USA. [Ma, Shuguo] Univ S Carolina, Dept Chem Engn, Columbia, SC 29208 USA. RP Wu, G (reprint author), Los Alamos Natl Lab, Mat Phys & Applicat Div, POB 1663, Los Alamos, NM 87545 USA. EM wugang@lanl.gov RI Wu, Gang/E-8536-2010; han, jiantao/F-8021-2010 OI Wu, Gang/0000-0003-4956-5208; han, jiantao/0000-0002-9509-3785 FU Los Alamos National Laboratory Early Career Laboratory-Directed Research and Development (LDRD) Program [20110483ER] FX We gratefully acknowledge the support of the Los Alamos National Laboratory Early Career Laboratory-Directed Research and Development (LDRD) Program (20110483ER) for this work. NR 50 TC 219 Z9 223 U1 40 U2 611 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 J9 ACS NANO JI ACS Nano PD NOV PY 2012 VL 6 IS 11 BP 9764 EP 9776 DI 10.1021/nn303275d PG 13 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 043CY UT WOS:000311521700046 PM 23036092 ER PT J AU Stavila, V Bhakta, RK Alam, TM Majzoub, EH Allendorf, MD AF Stavila, Vitalie Bhakta, Raghunandan K. Alam, Todd M. Majzoub, Eric H. Allendorf, Mark D. TI Reversible Hydrogen Storage by NaAlH4 Confined within a Titanium-Functionalized MOF-74(Mg) Nanoreactor SO ACS NANO LA English DT Article DE metal-organic frameworks; nanoreactors; metal hydrides; hydrogen storage; reversibility; nanoconfinement ID SODIUM ALANATE NANOPARTICLES; MELT INFILTRATION; ALUMINUM HYDRIDES; KINETICS; SIZE; THERMODYNAMICS; RELEASE; DEHYDROGENATION; NANOMATERIALS; CHEMISTRY AB We demonstrate that NaAlH4 confined within the nanopores of a titanium-functionalized metal-organic framework (MOF) template MOF-74(Mg) can reversibly store hydrogen with minimal loss of capacity. Hydride-infiltrated samples were synthesized by melt infiltration, achieving loadings up to 21 wt %. MOF-74(Mg) possesses one-dimensional, 12 angstrom channels lined with Mg atoms having open coordination sites, which can serve as sites for Ti catalyst stabilization. MOF-74(Mg) is stable under repeated hydrogen desorption and hydride regeneration cycles, allowing it to serve as a "nanoreactor". Confining NaAlH4 within these pores alters the decomposition pathway by eliminating the stable intermediate Na3AlH6 phase observed during bulk decomposition and proceeding directly to NaH, Al, and H-2, in agreement with theory. The onset of hydrogen desorption for both Ti-doped and undoped nano-NaAlN4@MOF-74(Mg) is similar to 50 degrees C, nearly 100 degrees C lower than bulk NaAlH4. However, the presence of titanium is not necessary for this increase In desorption kinetics but enables rehydriding to be almost fully reversible. Isothermal kinetic studies Indicate that the activation energy for H-2 desorption Is reduced from 793 kJ mol(-1) In bulk Ti-doped NaAlH4 to 574 kJ mol(-1) for nanoconfined NaAlH4. The structural properties of nano-NaAlH4@MOF-74(Mg) were probed using Na-23 and Al-27 solid-state MAS NMR, which indicates that the hydride Is not decomposed during Infiltration and that Al is present as tetrahedral AlH4 anions prior to desorption and as Al metal after desorption. Because of the highly ordered MOF structure and monodisperse pore; dimensions, our results allow key template features to be identified to ensure reversible, low-temperature hydrogen Storage. C1 [Stavila, Vitalie; Bhakta, Raghunandan K.; Allendorf, Mark D.] Sandia Natl Labs, Livermore, CA 94551 USA. [Alam, Todd M.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Majzoub, Eric H.] Univ Missouri, Ctr Nanosci, St Louis, MO 63130 USA. [Majzoub, Eric H.] Univ Missouri, Dept Phys & Astron, St Louis, MO 63130 USA. RP Stavila, V (reprint author), Sandia Natl Labs, Livermore, CA 94551 USA. EM vnstavi@sandia.gov; mdallen@sandia.gov RI Stavila, Vitalie/B-6464-2008 OI Stavila, Vitalie/0000-0003-0981-0432 FU U.S. DOE Hydrogen, Fuel Cells, and Infrastructure Technologies Program; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors acknowledge Dr. John Perry for assisting in the synthesis of MOF-74(Mg), and Jeffrey Chames for obtaining SEM/EDX data. We also thank Dr. Sean Maharrey for helpful discussions. This work was funded by the U.S. DOE Hydrogen, Fuel Cells, and Infrastructure Technologies Program. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 41 TC 45 Z9 45 U1 17 U2 287 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 J9 ACS NANO JI ACS Nano PD NOV PY 2012 VL 6 IS 11 BP 9807 EP 9817 DI 10.1021/nn304514c PG 11 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 043CY UT WOS:000311521700050 PM 23075161 ER PT J AU Zhou, H Rouha, M Feng, G Lee, SS Docherty, H Fenter, P Cummings, PT Fulvio, PF Dai, S McDonough, J Presser, V Gogotsi, Y AF Zhou, Hua Rouha, Michael Feng, Guang Lee, Sang Soo Docherty, Hugh Fenter, Paul Cummings, Peter T. Fulvio, Pasquale F. Dai, Sheng McDonough, John Presser, Volker Gogotsi, Yury TI Nanoscale Perturbations of Room Temperature Ionic Liquid Structure at Charged and Uncharged Interfaces SO ACS NANO LA English DT Article DE Room temperature ionic liquid; densification; epitaxial graphene; mica; charge overscreening; interfacial structure; X-ray reflectivity ID X-RAY REFLECTIVITY; CARBON NANOTUBES; DOUBLE-LAYER; ELECTROCHEMICAL CAPACITORS; EPITAXIAL GRAPHENE; MOLECULAR-DYNAMICS; SURFACE; SUPERCAPACITORS; IMIDAZOLIUM; SIMULATION AB The nanoscale interactions of room temperature ionic liquids (Rills) at uncharged (graphene) and charged (muscovite mica) solid surfaces were evaluated with high resolution X-ray interface scattering and fully atomistic molecular dynamics simulations. At uncharged graphene surfaces, the imidazolium-based RTIL {(bmim(+)][Tf2N-]) exhibits a mixed cation/anion layering with a strong Interfacial densification of the first RTIL layer. The first layer density observed via experiment is larger than that predicted by simulation and the apparent discrepancy can be understood with the inclusion of dominantly, image charge and pi-stacking interactions between the RTIL and the graphene sheet. In contrast the RTIL structure adjacent to the charged mica surface exhibits an alternating cation anion layering extending 3.5 nm Into the bulk fluid. The associated charge density profile demonstrates a pronounced charge overscreening (i.e., excess first-layer counterions with respect to the adjacent surface charge), highlighting the critical role of charge-Induced nanoscale correlations of the RTIL. These observations confirm key aspects of a predicted electric double layer structure from an analytical Landau-Ginzburg-type continuum theory incorporating ion correlation effects, and provide a new baseline for understanding the fundamental nanoscale response of RTILs at charged interfaces. C1 [Rouha, Michael; Feng, Guang; Docherty, Hugh; Cummings, Peter T.] Vanderbilt Univ, Dept Chem & Biomol Engn, Nashville, TN 37235 USA. [Cummings, Peter T.] Oak Ridge Natl Lab, Ctr Nanophase Mat, Oak Ridge, TN 37831 USA. [Fulvio, Pasquale F.; Dai, Sheng] Oak Ridge Natl Lab, Chem Sci Div, Oak Ridge, TN 37831 USA. [McDonough, John; Presser, Volker; Gogotsi, Yury] Drexel Univ, Dept Mat Sci & Engn, Philadelphia, PA 19104 USA. [McDonough, John; Presser, Volker; Gogotsi, Yury] Drexel Univ, AJ Drexel Nanotechnol Inst, Philadelphia, PA 19104 USA. [Zhou, Hua; Lee, Sang Soo; Fenter, Paul] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Zhou, H (reprint author), Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. EM hzhou@anl.gov; fenter@anl.gov RI Presser, Volker/F-1975-2010; Feng, Guang/D-8989-2011; Cummings, Peter/B-8762-2013; Gogotsi, Yury/B-2167-2008; Fulvio, Pasquale/B-2968-2014; Rouha, Michael/N-8187-2013; Dai, Sheng/K-8411-2015; OI Presser, Volker/0000-0003-2181-0590; Cummings, Peter/0000-0002-9766-2216; Gogotsi, Yury/0000-0001-9423-4032; Fulvio, Pasquale/0000-0001-7580-727X; Rouha, Michael/0000-0002-4227-4005; Dai, Sheng/0000-0002-8046-3931; Feng, Guang/0000-0001-6659-9181 FU Fluid Interface Reactions, Structures and Transport (FIRST) Center, an Energy Frontier Research Center; U.S. Department of Energy (DOE), Office of Science (SC), Office of Basic Energy Sciences (BES); DOE-SC-BES [DE-AC02-06CH11357]; DOE-SC [DE-AC02-05CH11231]; Alexander von Humboldt Foundation FX We thank especially Professor G. A. Baker at the Department of Chemistry in University of Missouri-Columbia for helping the synthesis of high purity [bmim+][Tf2N-]. This material is based upon work supported as part of the Fluid Interface Reactions, Structures and Transport (FIRST) Center, an Energy Frontier Research Center funded by the U.S. Department of Energy (DOE), Office of Science (SC), Office of Basic Energy Sciences (BES). Use of the beam lines 6ID and 33ID at the Advanced Photon Source was supported by DOE-SC-BES under Contract DE-AC02-06CH11357 to UChicago Argonne, LLC as operator of Argonne National Laboratory. This research used resources of the National Energy Research Scientific Computing Center, which is supported by DOE-SC under Contract No. DE-AC02-05CH11231, and the Palmetto cluster at Clemson University. V. Presser acknowledges financial support by the Alexander von Humboldt Foundation. NR 65 TC 66 Z9 66 U1 15 U2 242 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 J9 ACS NANO JI ACS Nano PD NOV PY 2012 VL 6 IS 11 BP 9818 EP 9827 DI 10.1021/nn303355b PG 10 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 043CY UT WOS:000311521700051 PM 23092400 ER PT J AU O'Hern, SC Stewart, CA Boutilier, MSH Idrobo, JC Bhaviripudi, S Das, SK Kong, J Laoui, T Atieh, M Karnik, R AF O'Hern, Sean C. Stewart, Cameron A. Boutilier, Michael S. H. Idrobo, Juan-Carlos Bhaviripudi, Sreekar Das, Sarit K. Kong, Jing Laoui, Tahar Atieh, Muataz Karnik, Rohit TI Selective Molecular Transport through Intrinsic Defects in a Single Layer of CVD Graphene SO ACS NANO LA English DT Article DE graphene membranes; nanofiltration; filtration; nanofluidics ID POROUS GRAPHENE; WATER; MEMBRANES; NUCLEATION; SEPARATION; OXIDATION; NANOPORES; GROWTH AB We report graphene composite membranes with nominal areas more than 25 mm(2) fabricated by transfer of a single layer of CVD graphene onto a porous polycarbonate substrate. A combination of pressure-driven and diffusive transport measurements provides evidence of size-selective transport of molecules through the membrane, which is attributed to the low-frequency occurrence of intrinsic 1-15 nm diameter pores in the CVD graphene. Our results present the first step toward the realization of practical membranes that use graphene as the selective material. C1 [O'Hern, Sean C.; Stewart, Cameron A.; Boutilier, Michael S. H.; Karnik, Rohit] MIT, Dept Mech Engn, Cambridge, MA 02139 USA. [Idrobo, Juan-Carlos] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Bhaviripudi, Sreekar; Kong, Jing] MIT, Dept Elect Engn & Comp Sci, Cambridge, MA 02139 USA. [Das, Sarit K.] Indian Inst Technol, Dept Mech Engn, Madras 600036, Tamil Nadu, India. [Laoui, Tahar; Atieh, Muataz] King Fahd Univ Petr & Minerals, Dept Mech Engn, Dhahran 31261, Saudi Arabia. [Laoui, Tahar; Atieh, Muataz] King Fahd Univ Petr & Minerals, Dept Chem Engn, Dhahran 31261, Saudi Arabia. RP Karnik, R (reprint author), MIT, Dept Mech Engn, Cambridge, MA 02139 USA. EM karnik@mit.edu RI Laoui, Tahar/B-6787-2015; Idrobo, Juan/H-4896-2015; OI Laoui, Tahar/0000-0002-9527-6610; Idrobo, Juan/0000-0001-7483-9034; ATIEH, MUATAZ/0000-0001-6805-0467 FU King Fahd University of Petroleum and Minerals in Dhahran, Saudi Arabia, through the Center for Clean Water and Clean Energy at MIT; KFUPM [R10-CW-09]; ORNL's Shared Research Equipment (ShaRE) User Program; Office of Basic Energy Sciences, U.S. Department of Energy; National Science Foundation [ECS-0335765] FX The authors would like to thank N. Hadjiconstantinou, T. Jain, and J. Lee for helpful discussions regarding this work and K. Mullen for assisting in graphene transfers. This work was funded by King Fahd University of Petroleum and Minerals in Dhahran, Saudi Arabia, through the Center for Clean Water and Clean Energy at MIT and KFUPM under project number R10-CW-09. The research was also supported by ORNL's Shared Research Equipment (ShaRE) User Program (J.C.I.), which is sponsored by the Office of Basic Energy Sciences, U.S. Department of Energy. Research was performed In part at the Center for Nanoscale Systems (CNS), a member of the National Nanotechnology Infrastructure Network, which is supported by the National Science Foundation under NSF award no. ECS-0335765. CNS is part of Harvard University. This research was also performed in part at the Center for Materials Science and Engineering at MIT. NR 37 TC 91 Z9 92 U1 8 U2 186 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 J9 ACS NANO JI ACS Nano PD NOV PY 2012 VL 6 IS 11 BP 10130 EP 10138 DI 10.1021/nn303869m PG 9 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 043CY UT WOS:000311521700086 PM 23030691 ER PT J AU Balke, N Tselev, A Arruda, TM Jesse, S Chu, YH Kalinin, SV AF Balke, Nina Tselev, Alexander Arruda, Thomas M. Jesse, Stephen Chu, Ying-Hao Kalinin, Sergei V. TI Probing Local Electromechanical Effects in Highly Conductive Electrolytes SO ACS NANO LA English DT Article DE scanning probe microscopy; liquid; ferroelectrics; electromechanics; piezoresponse force microscopy ID FERROELECTRIC THIN-FILMS; FORCE MICROSCOPY; DOMAIN-STRUCTURE; HIGH-RESOLUTION; POLARIZATION; CRYSTALS; POLYMERS; BEHAVIOR; SYSTEMS; STRAIN AB The functionality of a variety of materials and devices is strongly coupled with electromechanical effects which can be used to characterize their functionality. Of high interest is the investigation of these electromechanical effects on the nanoscale which can be achieved by using scanning probe microscopy. Here, an electrical bias is applied locally to the scanning probe tip, and the mechanical sample response is detected. In some applications with electromechanical phenomena, such as energy storage or for biological samples, a liquid environment is required to provide full functionality and sample stability. However, electromechanical sample characterization has mostly been applied in air or under vacuum due to the difficulties of applying local electric fields in a conductive environment. Here, we present a detailed study of piezoresponse force microscopy of ferroelectric samples in liquid environments as a model system for electromechanical effects in general. The ionic strength of the liquid is varied, and possibilities and limitations of the technique are explored. Numerical simulations are used to explain the observed phenomena and used to suggest strategies to work in liquid environments with high ionic strength. C1 [Balke, Nina; Tselev, Alexander; Arruda, Thomas M.; Jesse, Stephen; Kalinin, Sergei V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Chu, Ying-Hao] Natl Chiao Tung Univ, Dept Mat Sci & Engn, Hsinchu 30010, Taiwan. RP Balke, N (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM balken@ornl.gov RI Ying-Hao, Chu/A-4204-2008; Kalinin, Sergei/I-9096-2012; Arruda, Thomas/C-6134-2012; Tselev, Alexander/L-8579-2015; Balke, Nina/Q-2505-2015; Jesse, Stephen/D-3975-2016 OI Ying-Hao, Chu/0000-0002-3435-9084; Kalinin, Sergei/0000-0001-5354-6152; Arruda, Thomas/0000-0002-6165-2024; Tselev, Alexander/0000-0002-0098-6696; Balke, Nina/0000-0001-5865-5892; Jesse, Stephen/0000-0002-1168-8483 FU U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division through the Office of Science Early Career Research Program; National Science Council [NSC-101-2119-M-009-003-MY2]; Ministry of Education [MOE-ATU 101W961]; Center for Interdisciplinary Science of National Chiao Tung University FX The experiments were designed and performed supported by the U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division through the Office of Science Early Career Research Program. Instrumental capabilities and numerical calculations were provided and supported by the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. Samples were provided through the collaboration with the National Chiao Tung University supported by the National Science Council under Contract No. NSC-101-2119-M-009-003-MY2, Ministry of Education under Grant No. MOE-ATU 101W961, and Center for Interdisciplinary Science of National Chiao Tung University. NR 36 TC 2 Z9 2 U1 2 U2 78 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 J9 ACS NANO JI ACS Nano PD NOV PY 2012 VL 6 IS 11 BP 10139 EP 10146 DI 10.1021/nn3038868 PG 8 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 043CY UT WOS:000311521700087 PM 23106854 ER PT J AU Mai, JY Miller, H Hatch, AV AF Mai, Junyu Miller, Hanna Hatch, Anson V. TI Spatiotemporal Mapping of Concentration Polarization Induced pH Changes at Nanoconstrictions SO ACS NANO LA English DT Article DE nanoporous structure; pH mapping; concentration polarization; nanofluidic transport; preconcentration membrane; electrokinetic transport ID INTRACELLULAR PH; TRP CHANNELS; PROTEINS; PRECONCENTRATION; MEMBRANES; SELECTIVITY; MICROCHIPS; ENRICHMENT; TRANSPORT; PLATFORM AB Under an applied electric field, concentration polarization (CP) arises from ion permselectivity of most nanoporous materials and biological ion channels. We present novel methods to quantitatively assess CP-induced spatiotemporal changes of pH that may significantly impact transport dynamics, device functionality, and physicochemical properties of molecular analytes in devices with nanofluidic constrictions. We measured pH fluctuations of >1.5 pH units and changes extending over 100's of micrometers from nanoconstrictions. The degree of change depends on key system parameters including buffer composition, surface charge, and strength of electric field. The results highlight the importance of neglected contributions of pH changes, and the approach can aid characterization and manipulation of mass transport in nanofluidic systems. C1 [Mai, Junyu; Miller, Hanna; Hatch, Anson V.] Sandia Natl Labs, Dept Biotechnol & Bioengn, Livermore, CA 94551 USA. RP Hatch, AV (reprint author), Sandia Natl Labs, Dept Biotechnol & Bioengn, Livermore, CA 94551 USA. EM ahatch@sandia.gov FU Defense Threat Reduction Agency-Joint Science and Technology Office for Chemical and Biological Defense (IAA) [DTRA10027IA-3167]; Sandia's Laboratory Directed Research and Development Program; United States Department of Energy [DE-AC0494AL85000] FX We thank Dr. R. Meagher for insightful discussion. This project received support from the Defense Threat Reduction Agency-Joint Science and Technology Office for Chemical and Biological Defense (IAA number DTRA10027IA-3167) and from Sandia's Laboratory Directed Research and Development Program. Sandia is a multiprogram laboratory operated by Sandia Corp., a Lockheed Martin Co., for the United States Department of Energy under Contract DE-AC0494AL85000. NR 34 TC 10 Z9 10 U1 4 U2 42 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 J9 ACS NANO JI ACS Nano PD NOV PY 2012 VL 6 IS 11 BP 10206 EP 10215 DI 10.1021/nn304005p PG 10 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 043CY UT WOS:000311521700094 PM 23061977 ER PT J AU Singh, G Yager, KG Berry, B Kim, HC Karim, A AF Singh, Gurpreet Yager, Kevin G. Berry, Brian Kim, Ho-Cheol Karim, Alamgir TI Dynamic Thermal Field-Induced Gradient Soft-Shear for Highly Oriented Block Copolymer Thin Films SO ACS NANO LA English DT Article DE block copolymer; zone annealing; unidirectional nanostructures; thermal expansion induced shear; flexible substrate; PDMS template; hierarchical patterning ID SINGLE-LAYER FILMS; FACETED SURFACES; LITHOGRAPHY; ORDER; ORIENTATION; TEMPERATURE; TRANSITION; CYLINDERS; ARRAYS AB As demand for smaller, more powerful, and energy- efficient devices continues, conventional patterning technologies are pushing up against fundamental limits. Block copolymers (BCPs) are considered prime candidates for a potential solution via directed self-assembly of nanostructures. We Introduce here a facile directed self-assembly method to rapidly fabricate unidirectionally aligned BCP nanopattems at large scale, on rigid or flexible template-free substrates via a thermally induced dynamic gradient soft-shear field. A localized differential thermal expansion at the interface between a BCP film and a confining polydimethylsiloxane (PDMS) layer due to a dynamic thermal field imposes the gradient soft-shear field. PDMS undergoes directional expansion (along the annealing direction) in the heating zone and contracts back in the cooling zone, thus setting up a single cycle of oscillatory shear (maximum lateral shear stress similar to 12 x 10(4) Pa) in the system. We successfully apply this process to create unidirectional alignment of BCP thin films over a wide range of thicknesses (nm to mu m) and processing speeds (mu m/s to mm/s) using both a flat and patterned PDMS layer. Grazing incidence small-angle X-ray-scattering measurements show absolutely no sign of isotropic population and reveal >= 99% aligned orientational order with an angular spread Delta theta(twhm) <= 5 degrees (full width at half-maximum). This method may pave the way to practical industrial use of hierarchically patterned BCP nanostructures. C1 [Singh, Gurpreet; Karim, Alamgir] Univ Akron, Dept Polymer Engn, Akron, OH 44325 USA. [Yager, Kevin G.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Berry, Brian] Univ Arkansas, Dept Chem, Little Rock, AR 72204 USA. [Kim, Ho-Cheol] IBM Corp, Almaden Res Ctr, Div Res, San Jose, CA 95120 USA. RP Karim, A (reprint author), Univ Akron, Dept Polymer Engn, Akron, OH 44325 USA. EM alamgir@uakron.edu RI Yager, Kevin/F-9804-2011 OI Yager, Kevin/0000-0001-7745-2513 FU National Science Foundation (NSF), Division of Materials Research (DMR) [NSF DMR-1006421]; U.S:-Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX We would like to thank Prof. Shi-Qing Wang (The University of Akron), Dr. Christopher Stafford (NIST, USA), Dr. Diya Bandyopadhyay (The University of Akron), Dr. Manish Kulkarni (The University of Akron), and Arvind Modl (The University of Akron) for useful discussions. This CZA-SS research work was entirely supported by the National Science Foundation (NSF), Division of Materials Research (DMR), Grant NSF DMR-1006421. Supporting GISAXS was carried out in part at the National Synchrotron Light Source, and the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the U.S:-Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. NR 38 TC 60 Z9 61 U1 4 U2 79 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 J9 ACS NANO JI ACS Nano PD NOV PY 2012 VL 6 IS 11 BP 10335 EP 10342 DI 10.1021/nn304266f PG 8 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 043CY UT WOS:000311521700109 PM 23106286 ER PT J AU Holladay, JP Nisanian, M Williams, S Tuckfield, RC Kerr, R Jarrett, T Tannenbaum, L Holladay, SD Sharma, A Gogal, RM AF Holladay, Jeremy P. Nisanian, Mandy Williams, Susan Tuckfield, R. Cary Kerr, Richard Jarrett, Timothy Tannenbaum, Lawrence Holladay, Steven D. Sharma, Ajay Gogal, Robert M., Jr. TI Dosing of adult pigeons with as little as one #9 lead pellet caused severe delta-ALAD depression, suggesting potential adverse effects in wild populations SO ECOTOXICOLOGY LA English DT Article DE Lead; Avian; Ventriculus; Retention; delta-ALAD ID COEUR-DALENE RIVER; BLOOD CHARACTERISTICS; RISK-ASSESSMENT; MOURNING DOVES; CANADA GEESE; ACID; CALCIUM; BIRDS; SHOT; RETENTION AB Avian wildlife species commonly ingest lead (Pb) spent shot or bullet fragments as grit or mistakenly as food. In previous studies in our laboratory and others, the toxicity varied based on the diet as well as type and quantity of Pb ingested. In the current study, domestic pigeons were gavaged with 1, 2, or 3 Pb pellets and then followed with weekly radiographs and blood physiologic endpoints for 28 days. Pellet retention decreased by roughly 50 % per week as pellets were either absorbed or excreted, except for week 4 where pellet number no longer was diminished. Size of retained pellets visually decreased over retention time. Birds dosed with a single #9 pellet showed mean blood Pb levels over 80 times higher than those of the controls, verifying Pb pellet absorption from the gut. A single Pb pellet also reduced plasma delta-aminolevulinic acid dehydratase (delta-ALAD) activity by over 80 % compared to controls, suggesting the potential for population injury in Pb pellet-exposed pigeons. C1 [Holladay, Jeremy P.; Nisanian, Mandy; Kerr, Richard; Jarrett, Timothy; Holladay, Steven D.; Sharma, Ajay; Gogal, Robert M., Jr.] Univ Georgia, Coll Vet Med, Dept Biosci & Diagnost Imaging, Athens, GA 30602 USA. [Williams, Susan] Univ Georgia, Coll Vet Med, Dept Populat Hlth, Poultry Diagnost & Res Ctr, Athens, GA 30602 USA. [Tuckfield, R. Cary] Univ Georgia, Savannah River Ecol Lab, Athens, GA 30622 USA. [Tannenbaum, Lawrence] USA, Inst Publ Hlth, Aberdeen, MD 21010 USA. RP Gogal, RM (reprint author), Univ Georgia, Coll Vet Med, Dept Biosci & Diagnost Imaging, Athens, GA 30602 USA. EM rgogal@uga.edu FU Department of Defense, U.S. Army Institute for Public Health FX We wish to thank Mr. Danny Joe Humphrey of Color Pigeons for his advice on husbandry of the pigeons. We also wish to thank Dr. Carla Jarrett for assistance with bird restraint during the radiographs. We also wish to thank Mr. Michael Mottsinger and Mr. Brent Lovern of the Poultry Diagnostic Research Center at University of Georgia for care and maintenance of the birds. The study was funded by a grant from the Department of Defense, U.S. Army Institute for Public Health. NR 29 TC 4 Z9 4 U1 1 U2 27 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0963-9292 J9 ECOTOXICOLOGY JI Ecotoxicology PD NOV PY 2012 VL 21 IS 8 BP 2331 EP 2337 DI 10.1007/s10646-012-0989-x PG 7 WC Ecology; Environmental Sciences; Toxicology SC Environmental Sciences & Ecology; Toxicology GA 058WG UT WOS:000312664900023 PM 22903291 ER PT J AU Yun, K Luck, R Mago, PJ Cho, H AF Yun, Kyungtae Luck, Rogelio Mago, Pedro J. Cho, Heejin TI Building hourly thermal load prediction using an indexed ARX model SO ENERGY AND BUILDINGS LA English DT Article DE Building thermal load prediction; Linear regression model; Autoregressive model ID COOLING LOAD; REGRESSION AB This paper introduces an easily implementable and computationally efficient, ARX (autoregressive with exogenous, i.e., external, inputs) time and temperature indexed model for 1 h ahead building thermal load prediction. Time and temperature indexing implies that different sets of coefficients are used in the predictive equation depending on the time of the day or the ambient temperature. The indexing and proposed structure of the model follows physically motivated interpretations of the loading conditions and thermal response of the building. One of the main contributions of the proposed model is that it allows determining the dominant factors that affect the thermal load at a given time. A free and widely adopted building energy and thermal load simulation program from the U.S. Department of Energy is used to determine the prediction accuracy of the proposed model on several different benchmark-building types: a small office building, a medium office building, a midrise apartment, and a high-rise apartment. (C) 2012 Elsevier B.V. All rights reserved. C1 [Yun, Kyungtae; Luck, Rogelio; Mago, Pedro J.] Mississippi State Univ, Dept Mech Engn, Mississippi State, MS 39762 USA. [Cho, Heejin] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Yun, K (reprint author), Mississippi State Univ, Dept Mech Engn, 210 Carpenter Engn Bldg,POB ME, Mississippi State, MS 39762 USA. EM ky57@msstate.edu OI Cho, Heejin/0000-0003-2789-510X NR 25 TC 18 Z9 18 U1 2 U2 6 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0378-7788 J9 ENERG BUILDINGS JI Energy Build. PD NOV PY 2012 VL 54 BP 225 EP 233 DI 10.1016/j.enbuild.2012.08.007 PG 9 WC Construction & Building Technology; Energy & Fuels; Engineering, Civil SC Construction & Building Technology; Energy & Fuels; Engineering GA 059ZU UT WOS:000312745200026 ER PT J AU Hart, R Goudey, H Arasteh, D Curcija, DC AF Hart, Robert Goudey, Howdy Arasteh, Dariush Curcija, D. Charlie TI Thermal performance impacts of center-of-glass deflections in installed insulating glazing units SO ENERGY AND BUILDINGS LA English DT Article DE Insulating glass unit; U-factor; Thermal transmittance; Thermal performance; Deflection; Concave; Convex; Gap; Field test AB This study examines the thermal performance impact of center-of-glass (COG) deflections in double- and triple-pane insulating glass units (IGUs) installed at several locations throughout the U.S. Deflection was measured during summer and winter temperatures; the results show that outdoor temperature variations can be represented a linear change in COG gap width in double- and triple-pane IGUs within the temperature ranges measured. However, the summer-winter temperature-induced deflection is similar in magnitude to the observed spread in COG deflection of similar units at the same temperature, which suggests that factors other than temperature are of equal importance in determining the in situ deflection of windows. The effect of deflection on thermal performance depends on the IGU's designed gap. Units constructed with smaller-than-optimal gaps often exhibit significant U-factor change due to temperature-induced reduction in gap width. This effect is particularly problematic in high-performance triple glazing where small gap dimension changes can have a large impact on performance. (C) 2012 Elsevier B.V. All rights reserved. C1 [Hart, Robert; Goudey, Howdy; Arasteh, Dariush; Curcija, D. Charlie] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Windows & Daylighting Grp, Berkeley, CA 94720 USA. RP Hart, R (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Windows & Daylighting Grp, 1 Cyclotron Rd,Mail Stop 90R3111, Berkeley, CA 94720 USA. EM rghart@lbl.gov FU U.S. Department of Energy [DE-AC02-05CH11231] FX Thanks to Robert Clear for his valuable insight and support in the statistical analysis. This work was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Building Technologies Program, of the U.S. Department of Energy under Contract no. DE-AC02-05CH11231. NR 8 TC 3 Z9 3 U1 2 U2 9 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0378-7788 J9 ENERG BUILDINGS JI Energy Build. PD NOV PY 2012 VL 54 BP 453 EP 460 DI 10.1016/j.enbuild.2012.06.026 PG 8 WC Construction & Building Technology; Energy & Fuels; Engineering, Civil SC Construction & Building Technology; Energy & Fuels; Engineering GA 059ZU UT WOS:000312745200049 ER PT J AU Mishra, U Torn, MS Masanet, E Ogle, SM AF Mishra, Umakant Torn, Margaret S. Masanet, Eric Ogle, Stephen M. TI Improving regional soil carbon inventories: Combining the IPCC carbon inventory method with regression kriging SO GEODERMA LA English DT Article DE Soil carbon inventory; Intergovernmental panel on climate change; Regression kriging; No-tillage ID ORGANIC-CARBON; UNCERTAINTY ANALYSIS; MANAGEMENT IMPACTS; AGRICULTURAL LANDS; C SEQUESTRATION; TILLAGE; SCALE; PREDICTION; STORAGE; MATTER AB Regional assessments of change in soil organic carbon (SOC) stocks due to land-use change are essential for supporting policy and management decisions related to greenhouse gas emissions and mitigation through carbon sequestration in soils. We have developed an improved approach by integrating geostatistical techniques with the Intergovernmental Panel on Climate Change (IPCC) carbon inventory approach to assess the impact of no-till management and crop-residue retention on SOC changes at a regional scale. Specifically, the improved approach utilizes regression kriging (RK) to estimate reference carbon stocks for the IPCC method. In our case study, we compared the results from the RI( method with a simple averaging (SA) method to derive the reference stocks as implemented in the Tier 2 IPCC approach, for a seven state area of the Midwestern United States. Using this improved method, we predict that eliminating tillage and retaining crop residues on all croplands of the study area would result in 11,735 Gg C yr(-1) sequestration for 20 years in the top 30 cm of the soil profile. Most cropland area would sequester 02-0.75 Mg C ha(-1) yr(-1). However, at a few places, the predicted rate of sequestration was more than 0.75 Mg C ha(-1) yr(-1), with an upper limit of 1.1 Mg C ha(-1) yr(-1). The highest rates of carbon accumulation were associated with favorable environmental conditions, such as lower slope positions and cold, temperate, moist climates. Validating predicted SOC change at 18 sites with varying soil types and environmental conditions showed that the RK approach to estimate reference carbon stocks decreased global prediction errors by 45% relative to the default reference values. The increase in prediction accuracy was due to using spatially varying SOC stocks rather than simple data averaging to derive reference SOC values. The uncertainty analysis demonstrated that there was more precision in the results from the RK approach in comparison to the results from the SA approach. These results suggest that improved geostatistical approach is a promising technique for improving soil carbon inventories that utilize the IPCC method, and will provide more precise results for informing public policy and management decisions while retaining ease of application. (C) 2012 Elsevier B.V. All rights reserved. C1 [Mishra, Umakant; Torn, Margaret S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Masanet, Eric] Northwestern Univ, Dept Mech Engn, Evanston, IL 60208 USA. [Ogle, Stephen M.] Colorado State Univ, Nat Resource Ecol Lab, Ft Collins, CO 80523 USA. RP Mishra, U (reprint author), Argonne Natl Lab, Div Environm Sci, 9700 S Cass Ave,Bldg 240, Argonne, IL 60439 USA. EM umishra@anl.gov RI Masanet, Eric /I-5649-2012; Mishra, Umakant/H-8128-2013; Torn, Margaret/D-2305-2015; OI Ogle, Stephen/0000-0003-1899-7446 FU Energy Biosciences Institute, University of California Berkeley; Office of Biological and Environmental Research, Climate and Environmental Science Division, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This study was funded by the Energy Biosciences Institute, University of California Berkeley and Office of Biological and Environmental Research, Climate and Environmental Science Division, of the U.S. Department of Energy under contract no. DE-AC02-05CH11231 to Lawrence Berkeley National Laboratory. NR 36 TC 11 Z9 12 U1 4 U2 52 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0016-7061 J9 GEODERMA JI Geoderma PD NOV PY 2012 VL 189 BP 288 EP 295 DI 10.1016/j.geoderma.2012.06.022 PG 8 WC Soil Science SC Agriculture GA 047XX UT WOS:000311875900033 ER PT J AU Zhang, G Harichandran, RS Ramuhalli, P AF Zhang, Gang Harichandran, Ronald S. Ramuhalli, Pradeep TI Automatic Delamination Detection of Concrete Bridge Decks Using Impact Signals SO JOURNAL OF BRIDGE ENGINEERING LA English DT Article DE Delamination; Concrete bridge decks; Acoustic NDE; Impact signals AB Delamination of the concrete cover above the upper reinforcing bars is a common problem in concrete bridge decks. Acoustic non-destructive evaluation is widely used to detect such delamination because of its low cost, fast speed, and ease of implementation. The accuracy of traditional acoustic approaches is dependent on the level of ambient noise, and the detection process is highly subjective. An automatic impact-based delamination detection (AIDD) system is described in this paper. In this system, the traffic noise is eliminated by a modified version of independent component analysis. Mel-frequency cepstral coefficients are then used as features for detection to eliminate subjectivity. The delamination detection is performed by a radial basis function neural network. The AIDD system was developed using mixed-language programming in MATLAB, LabVIEW, and C++. The performance of the system was evaluated using data from two bridges, and the results were satisfactory. DOI: 10.1061/(ASCE)BE.1943-5592.0000326. (C) 2012 American Society of Civil Engineers. C1 [Zhang, Gang] Fed Highway Adm, Mclean, VA 22101 USA. [Harichandran, Ronald S.] Univ New Haven, Tagliatela Coll Engn, West Haven, CT 06516 USA. [Harichandran, Ronald S.] Michigan State Univ, Dept Civil & Environm Engn, E Lansing, MI 48824 USA. [Ramuhalli, Pradeep] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Zhang, G (reprint author), Fed Highway Adm, 6300 Georgetown Pike, Mclean, VA 22101 USA. EM civilzhang@gmail.com OI Ramuhalli, Pradeep/0000-0001-6372-1743 FU Michigan Department of Transportation (MDOT) FX This research was sponsored by the Michigan Department of Transportation (MDOT). The authors would like to thank the project manager, Steve Kahl, and all members of the research advisory panel for their input related to this research. The opinions, findings, conclusions, and recommendations presented herein are those of the authors alone and do not necessarily represent the views and opinions of MDOT. NR 22 TC 0 Z9 0 U1 0 U2 3 PU ASCE-AMER SOC CIVIL ENGINEERS PI RESTON PA 1801 ALEXANDER BELL DR, RESTON, VA 20191-4400 USA SN 1084-0702 J9 J BRIDGE ENG JI J. Bridge Eng. PD NOV-DEC PY 2012 VL 17 IS 6 SI SI BP 951 EP 954 DI 10.1061/(ASCE)BE.1943-5592.0000326 PG 4 WC Engineering, Civil SC Engineering GA 058UX UT WOS:000312661300014 ER PT J AU Silin, D Kneafsey, T AF Silin, D. Kneafsey, T. TI Shale Gas: Nanometer-Scale Observations and Well Modelling SO JOURNAL OF CANADIAN PETROLEUM TECHNOLOGY LA English DT Article; Proceedings Paper CT Canadian Unconventional Resources and International Petroleum Conference CY NOV 15-17, 2011 CL Calgary, CANADA ID ADSORPTION HYSTERESIS; BARNETT SHALE; NATURAL-GAS; NANOPORES; SYSTEMS; STORAGE AB Our studies of the underlying fundamental gas-recovery mechanisms from shale gas are motivated by expectations of the increasing role of shale gas in national energy portfolios worldwide. We use pore-scale analysis of reservoir shale samples to identify critical parameters to be employed in a gas-flow model used to evaluate well-production data. We exploit a number of 3D-imaging technologies to study the complexity of shale pore structure: from low-resolution X-ray computed tomography (CT) to focused ion beam and scanning electron microscopy (FIB/SEM). We observe that heterogeneity is present at all scales. The CT data show fractures, thin layers, and density heterogeneity. The nanometer-scale-resolution FIB/SEM images show that various mineral inclusions, clays, and organic matter are dispersed within a volume of few-hundred mu m(3). Samples from different regions differ sharply in the shape, size, and distribution of pores, solid grains, and the presence of organic matter. Although the samples have clearly distinguishable signatures related to the regions of origin, extremely low permeability is a common feature. This and other pore-scale observations suggest a bounded-stimulated-domain model of a horizontal well within fractured shale that accounts for both compression and adsorption gas storage. Using the method of integral relations, we obtain an analytical formula approximating the solution to the nonlinear pressure diffusion equation. This formula makes fast and simple evaluation of well production possible without resorting to complex computations. It defines a decline curve, which predicts two stages of production. During the early stage, the production rate declines with the reciprocal of the square root of time, whereas later, the rate declines exponentially. The model has been verified by successfully matching monthly production data from a number of shale-gas wells collected over several years of operation. Under appropriate conditions, scaling can collapse the data from multiple wells on a single type curve. Pore-scale image analysis and the mesoscale model suggest a dimensionless adsorption-storage factor (ASF) to characterize the relative contributions of compression and adsorption gas storage. C1 [Silin, D.; Kneafsey, T.] Lawrence Berkeley Natl Lab, Berkeley, CA USA. RI Kneafsey, Timothy/H-7412-2014 OI Kneafsey, Timothy/0000-0002-3926-8587 NR 37 TC 14 Z9 16 U1 1 U2 75 PU SPE-SOC PETROLEUM ENGINEERS, CANADA PI CALGARY PA 500-5 AVE SW, STE 425, CALGARY, ALBERTA T2P 3L5, CANADA SN 0021-9487 EI 2156-4663 J9 J CAN PETROL TECHNOL JI J. Can. Pet. Technol. PD NOV PY 2012 VL 51 IS 6 BP 464 EP 475 PG 12 WC Energy & Fuels; Engineering, Chemical; Engineering, Petroleum SC Energy & Fuels; Engineering GA 056HJ UT WOS:000312478700006 ER PT J AU Wang, ZG Gao, F AF Wang, Zhiguo Gao, Fei TI Defects and Doping in One-Dimensional SiC Nanostructures SO JOURNAL OF COMPUTATIONAL AND THEORETICAL NANOSCIENCE LA English DT Review DE SiC Nanowire; SiC Nanotube; One-Dimensional Nanostructure; Defects; Doping; Amorphous Coating; Twinning ID CHEMICAL-VAPOR-DEPOSITION; SILICON-CARBIDE NANOSTRUCTURES; ELECTRICAL-PROPERTIES; CARBON NANOTUBES; 1ST PRINCIPLES; NANOWIRES; NANORODS; BORON; GROWTH; PHOTOLUMINESCENCE AB The unique properties of one-dimensional (1D) SiC nanostructures make them to be potential applications in novel nanoscale devices. Considerable efforts have been made in fabricating SiC nanostructures, and 1D SiC nanostructures, such as nanotube, nanowire, nanorods, and nanocalble, have been synthesized successfully. Theoretical calculations show that 1D nanostructures have outstanding electronic and mechanical properties. Defects and doping are inevitable during processing and lead to many practical applications. In this paper, the defects and doping effects in 1D SiC nanostuctures are reviewed. Both quantum size and surface effects are not favorable for efficient doping in low-dimensional systems. The ionization energy of dopants increases with increasing the diameter of the nanostructures. The twinning and amorphous coating have a great effect on the mechanical behavior of 1D SiC nanowires. Amorphous layer coating can induce brittle to ductile transition in SiC nanowires, and decreases the critical yield stress and Young's modulus, whereas the critical strain of the nanowires can be enhanced by twin-stacking faults. C1 [Wang, Zhiguo] Univ Elect Sci & Technol China, Dept Appl Phys, Chengdu 610054, Peoples R China. [Wang, Zhiguo; Gao, Fei] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. RP Wang, ZG (reprint author), Univ Elect Sci & Technol China, Dept Appl Phys, Chengdu 610054, Peoples R China. RI Wang, Zhiguo/B-7132-2009 FU Young Scientists Foundation of Sichuan [09ZQ026-029]; Division of Materials Sciences and Engineering, Office of Basic Energy Sciences, US Department of Energy (DOE) [DE-AC05-76RL01830] FX Z. Wang was financially supported by the Young Scientists Foundation of Sichuan (09ZQ026-029). F. Gao was supported by the Division of Materials Sciences and Engineering, Office of Basic Energy Sciences, US Department of Energy (DOE) under Contract DE-AC05-76RL01830. NR 78 TC 1 Z9 1 U1 4 U2 77 PU AMER SCIENTIFIC PUBLISHERS PI VALENCIA PA 26650 THE OLD RD, STE 208, VALENCIA, CA 91381-0751 USA SN 1546-1955 EI 1546-1963 J9 J COMPUT THEOR NANOS JI J. Comput. Theor. Nanosci. PD NOV PY 2012 VL 9 IS 11 SI SI BP 1967 EP 1974 DI 10.1166/jctn.2012.2602 PG 8 WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 058GB UT WOS:000312621000010 ER PT J AU Zhang, YF Huang, HC AF Zhang, Yongfeng Huang, Hanchen TI Design of Twin Structures in SiC Nanowires SO JOURNAL OF COMPUTATIONAL AND THEORETICAL NANOSCIENCE LA English DT Review DE Silicon Carbide; Nanowire; Twin Boundary; Mechanical Property; Electronic Property ID SILICON-CARBIDE NANOWIRES; LOW-TEMPERATURE; MECHANISM; NANOSTRUCTURES; GROWTH; ELASTICITY; PLASTICITY; BOUNDARIES; STABILITY; STRENGTH AB With covalent bonding, SiC has high mechanical strength and a large energy gap in electronic band structure. Nanoscale SiC, in the form of nanowires, has increased mechanical toughness and variable band gaps. Further, introduction of twin boundaries into cubic SiC nanowires can result in improvement in both mechanical and electronic properties. This review presents effects of twin boundaries on properties of cubic SiC nanowires, including mechanical and electronic properties. Further, this review presents recent developments in introducing twin boundaries into cubic SiC nanowires, controllably and uncontrollably. C1 [Zhang, Yongfeng; Huang, Hanchen] Univ Connecticut, Dept Mech Engn, Storrs, CT 06269 USA. RP Zhang, YF (reprint author), Idaho Natl Lab, POB 1625, Idaho Falls, ID 83415 USA. RI Huang, Hanchen/A-9323-2008 FU Department of Energy Office of Basic Energy Sciences [DE-FG02-09ER46562]; Defense Threat Reduction Agency [HDTRA1-09-1-0027] FX The authors acknowledge financial support from the Department of Energy Office of Basic Energy Sciences (DE-FG02-09ER46562) and Defense Threat Reduction Agency (HDTRA1-09-1-0027). NR 43 TC 0 Z9 0 U1 1 U2 35 PU AMER SCIENTIFIC PUBLISHERS PI VALENCIA PA 26650 THE OLD RD, STE 208, VALENCIA, CA 91381-0751 USA SN 1546-1955 J9 J COMPUT THEOR NANOS JI J. Comput. Theor. Nanosci. PD NOV PY 2012 VL 9 IS 11 SI SI BP 1975 EP 1979 DI 10.1166/jctn.2012.2603 PG 5 WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 058GB UT WOS:000312621000011 ER PT J AU Gasperikova, E Hubbard, SS Watson, DB Baker, GS Peterson, JE Kowalsky, MB Smith, M Brooks, S AF Gasperikova, Erika Hubbard, Susan S. Watson, David B. Baker, Gregory S. Peterson, John E. Kowalsky, Michael B. Smith, Meagan Brooks, Scott TI Long-term electrical resistivity monitoring of recharge-induced contaminant plume behavior SO JOURNAL OF CONTAMINANT HYDROLOGY LA English DT Article DE Electrical resistivity; Contaminant plume; Time-lapse monitoring; Nitrate; Rainfall ID SOLUTE TRANSPORT; RESISTANCE TOMOGRAPHY; VADOSE ZONE; INVERSION; SCALE; TIME; ERT; GROUNDWATER; SUBSURFACE; MODELS AB Geophysical measurements, and electrical resistivity tomography (ERT) data in particular, are sensitive to properties that are related (directly or indirectly) to hydrological processes. The challenge is in extracting information from geophysical data at a relevant scale that can be used to gain insight about subsurface behavior and to parameterize or validate flow and transport models. Here, we consider the use of ERT data for examining the impact of recharge on subsurface contamination at the S-3 ponds of the Oak Ridge Integrated Field Research Challenge (IFRC) site in Tennessee. A large dataset of time-lapse cross-well and surface ERT data, collected at the site over a period of 12 months, is used to study time variations in resistivity due to changes in total dissolved solids (primarily nitrate). The electrical resistivity distributions recovered from cross-well and surface ERT data agrees well, and both of these datasets can be used to interpret spatiotemporal variations in subsurface nitrate concentrations due to rainfall, although the sensitivity of the electrical resistivity response to dilution varies with nitrate concentration. Using the time-lapse surface ERT data interpreted in terms of nitrate concentrations, we find that the subsurface nitrate concentration at this site varies as a function of spatial position, episodic heavy rainstorms (versus seasonal and annual fluctuations), and antecedent rainfall history. These results suggest that the surface ERT monitoring approach is potentially useful for examining subsurface plume responses to recharge over field-relevant scales. Published by Elsevier B.V. C1 [Gasperikova, Erika; Hubbard, Susan S.; Peterson, John E.; Kowalsky, Michael B.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Baker, Gregory S.; Smith, Meagan] Univ Tennessee, Dept Earth & Planetary Sci, Knoxville, IN 37996 USA. [Watson, David B.; Brooks, Scott] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Gasperikova, E (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd,MS 74R0120, Berkeley, CA 94720 USA. EM egasperikova@lbl.gov; sshubbard@lbl.gov; watsondb@ornl.gov; gbaker@tennessee.edu; jepeterson@lbl.gov; mbkowalsky@lbl.gov; msmith79@utk.edu; brookssc@ornl.gov RI Gasperikova, Erika/D-1117-2015; Hubbard, Susan/E-9508-2010; Watson, David/C-3256-2016 OI Gasperikova, Erika/0000-0003-1553-4569; Watson, David/0000-0002-4972-4136 FU U.S. Department of Energy [DE-AC02-05CH11231]; U.S. DOE Office of Biological and Environmental Research as part of the Oak Ridge National Laboratory IFRC Study FX This work was supported by the U.S. Department of Energy, Contract No. DE-AC02-05CH11231 and by the Subsurface Biogeochemical Research Program of the U.S. DOE Office of Biological and Environmental Research as part of the Oak Ridge National Laboratory IFRC Study. The authors would like to thank Marcella Mueller (ORNL) for assistance with the hydrogeochemical data, and two anonymous reviewers for suggestions and comments that helped us to improve this manuscript. NR 52 TC 13 Z9 15 U1 1 U2 33 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0169-7722 EI 1873-6009 J9 J CONTAM HYDROL JI J. Contam. Hydrol. PD NOV PY 2012 VL 142 BP 33 EP 49 DI 10.1016/j.jconhyd.2012.09.007 PG 17 WC Environmental Sciences; Geosciences, Multidisciplinary; Water Resources SC Environmental Sciences & Ecology; Geology; Water Resources GA 060CB UT WOS:000312753000004 PM 23103519 ER PT J AU Aad, G Abajyan, T Abbott, B Abdallah, J Khalek, SA Abdelalim, AA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Acharya, BS Adamczyk, L Adams, DL Addy, TN Adelman, J Adomeit, S Adragna, P Adye, T Aefsky, S Aguilar-Saavedra, JA Agustoni, M Aharrouche, M Ahlen, SP Ahles, F Ahmad, A Ahsan, M Aielli, G Akdogan, T Akesson, TPA Akimoto, G Akimov, AV Alam, MS Alam, MA Albert, J Albrand, S Aleksa, M Aleksandrov, IN Alessandria, F Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Aliev, M Alimonti, G Alison, J Allbrooke, BMM Allport, PP Allwood-Spiers, SE Almond, J Aloisio, A Alon, R Alonso, A Alonso, F Altheimer, AD Gonzalez, BA Alviggi, MG Amako, K Amelung, C Ammosov, VV Amorim, A Amram, N Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Anduaga, XS Anger, P Angerami, A Anghinolfi, F Anisenkov, A Anjos, N Annovi, A Antonaki, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Aoun, S Bella, LA Apolle, R Arabidze, G Aracena, I Arai, Y Arce, ATH Arfaoui, S Arguin, JF Arik, E Arik, M Armbruster, AJ Arnaez, O Arnal, V Arnault, C Artamonov, A Artoni, G Arutinov, D Asai, S Asfandiyarov, R Ask, S Asman, B Asquith, L Assamagan, K Astbury, A Atkinson, M Aubert, B Auge, E Augsten, K Aurousseau, M Avolio, G Avramidou, R Axen, D Azuelos, G Azuma, Y Baak, MA Baccaglioni, G Bacci, C Bach, AM Bachacou, H Bachas, K Backes, M Backhaus, M Badescu, E Bagnaia, P Bahinipati, S Bai, Y Bailey, DC Bain, T Baines, JT Baker, OK Baker, MD Baker, S Banas, E Banerjee, P Banerjee, S Banfi, D Bangert, A Bansal, V Bansil, HS Barak, L Baranov, SP Galtieri, AB Barber, T Barberio, EL Barberis, D Barbero, M Bardin, DY Barillari, T Barisonzi, M Barklow, T Barlow, N Barnett, BM Barnett, RM Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Barrillon, P Bartoldus, R Barton, AE Bartsch, V Basye, A Bates, RL Batkova, L Batley, JR Battaglia, A Battistin, M Bauer, F Bawa, HS Beale, S Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, AK Becker, S Beckingham, M Becks, KH Beddall, AJ Beddall, A Bedikian, S Bednyakov, VA Bee, CP Beemster, LJ Begel, M Harpaz, SB Beimforde, M Belanger-Champagne, C Bell, PJ Bell, WH Bella, G Bellagamba, L Bellina, F Bellomo, M Belloni, A Beloborodova, O Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Benoit, M Bensinger, JR Benslama, K Bentvelsen, S Berge, D Kuutmann, EB Berger, N Berghaus, F Berglund, E Beringer, J Bernat, P Bernhard, R Bernius, C Berry, T Bertella, C Bertin, A Bertolucci, F Besana, MI Besjes, GJ Besson, N Bethke, S Bhimji, W Bianchi, RM Bianco, M Biebel, O Bieniek, SP Bierwagen, K Biesiada, J Biglietti, M Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Biscarat, C Bittner, B Black, KM Blair, RE Blanchard, JB Blanchot, G Blazek, T Bloch, I Blocker, C Blocki, J Blondel, A Blum, W Blumenschein, U Bobbink, GJ Bobrovnikov, VB Bocchetta, SS Bocci, A Boddy, CR Boehler, M Boek, J Boelaert, N Bogaerts, JA Bogdanchikov, A Bogouch, A Bohm, C Bohm, J Boisvert, V Bold, T Boldea, V Bolnet, NM Bomben, M Bona, M Boonekamp, M Bordoni, S Borer, C Borisov, A Borissov, G Borjanovic, I Borri, M Borroni, S Bortolotto, V Bos, K Boscherini, D Bosman, M Boterenbrood, H Bouchami, J Boudreau, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boveia, A Boyd, J Boyko, IR Bozovic-Jelisavcic, I Bracinik, J Branchini, P Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Brazzale, SF Brelier, B Bremer, J Brendlinger, K Brenner, R Bressler, S Britton, D Brochu, FM Brock, I Brock, R Broggi, F Bromberg, C Bronner, J Brooijmans, G Brooks, T Brooks, WK Brown, G Brown, H de Renstrom, PAB Bruncko, D Bruneliere, R Brunet, S Bruni, A Bruni, G Bruschi, M Buanes, T Buat, Q Bucci, F Buchanan, J Buchholz, P Buckingham, RM Buckley, AG Buda, SI Budagov, IA Budick, B Buscher, V Bugge, L Bulekov, O Bundock, AC Bunse, M Buran, T Burckhart, H Burdin, S Burgess, T Burke, S Busato, E Bussey, P Buszello, CP Butler, B Butler, JM Buttar, CM Butterworth, JM Buttinger, W Urban, SC Caforio, D Cakir, O Calafiura, P Calderini, G Calfayan, P Calkins, R Caloba, LP Caloi, R Calvet, D Calvet, S Toro, RC Camarri, P Cameron, D Caminada, LM Armadans, RC Campana, S Campanelli, M Canale, V Canelli, F Canepa, A Cantero, J Cantrill, R Capasso, L Garrido, MDMC Caprini, I Caprini, M Capriotti, D Capua, M Caputo, R Cardarelli, R Carli, T Carlino, G Carminati, L Caron, B Caron, S Carquin, E Montoya, GDC Carter, AA Carter, JR Carvalho, J Casadei, D Casado, MP Cascella, M Caso, C Hernandez, AMC Castaneda-Miranda, E Gimenez, VC Castro, NF Cataldi, G Catastini, P Catinaccio, A Catmore, JR Cattai, A Cattani, G Caughron, S Cavaliere, V Cavalleri, P Cavalli, D Cavalli-Sforza, M Cavasinni, V Ceradini, F Cerqueira, AS Cerri, A Cerrito, L Cerutti, F Cetin, SA Chafaq, A Chakraborty, D Chalupkova, I Chan, K Chang, P Chapleau, B Chapman, JD Chapman, JW Chareyre, E Charlton, DG Chavda, V Barajas, CAC Cheatham, S Chekanov, S Chekulaev, SV Chelkov, GA Chelstowska, MA Chen, C Chen, H Chen, S Chen, X Chen, Y Cheplakov, A El Moursli, RC Chernyatin, V Cheu, E Cheung, SL Chevalier, L Chiefari, G Chikovani, L Childers, JT Chilingarov, A Chiodini, G Chisholm, AS Chislett, RT Chitan, A Chizhov, MV Choudalakis, G Chouridou, S Christidi, IA Christov, A Chromek-Burckhart, D Chu, ML Chudoba, J Ciapetti, G Ciftci, AK Ciftci, R Cinca, D Cindro, V Ciocca, C Ciocio, A Cirilli, M Cirkovic, P Citterio, M Ciubancan, M Clark, A Clark, PJ Clarke, RN Cleland, W Clemens, JC Clement, B Clement, C Coadou, Y Cobal, M Coccaro, A Cochran, J Coffey, L Cogan, JG Coggeshall, J Cogneras, E Colas, J Cole, S Colijn, AP Collins, NJ Collins-Tooth, C Collot, J Colombo, T Colon, G Muino, PC Coniavitis, E Conidi, MC Consonni, SM Consorti, V Constantinescu, S Conta, C Conti, G Conventi, F Cooke, M Cooper, BD Cooper-Sarkar, AM Copic, K Cornelissen, T Corradi, M Corriveau, F Cortes-Gonzalez, A Cortiana, G Costa, G Costa, MJ Costanzo, D Cote, D Courneyea, L Cowan, G Cowden, C Cox, BE Cranmer, K Crescioli, F Cristinziani, M Crosetti, G Crepe-Renaudin, S Cuciuc, CM Almenar, CC Donszelmann, TC Curatolo, M Curtis, CJ Cuthbert, C Cwetanski, P Czirr, H Czodrowski, P Czyczula, Z D'Auria, S D'Onofrio, M D'Orazio, A De Sousa, MJDS Da Via, C Dabrowski, W Dafinca, A Dai, T Dallapiccola, C Dam, M Dameri, M Damiani, DS Danielsson, HO Dao, V Darbo, G Darlea, GL Dassoulas, JA Davey, W Davidek, T Davidson, N Davidson, R Davies, E Davies, M Davignon, O Davison, AR Davygora, Y Dawe, E Dawson, I Daya-Ishmukhametova, RK De, K de Asmundis, R De Castro, S De Cecco, S de Graat, J De Groot, N de Jong, P De la Taille, C De la Torre, H De Lorenzi, F de Mora, L De Nooij, L De Pedis, D De Salvo, A De Sanctis, U De Santo, A De Regie, JBD De Zorzi, G Dearnaley, WJ Debbe, R Debenedetti, C Dechenaux, B Dedovich, DV Degenhardt, J Del Papa, C Del Peso, J Del Prete, T Delemontex, T Deliyergiyev, M Dell'Acqua, A Dell'Asta, L Della Pietra, M della Volpe, D Delmastro, M Delsart, PA Deluca, C Demers, S Demichev, M Demirkoz, B Deng, J Denisov, SP Derendarz, D Derkaoui, JE Derue, F Dervan, P Desch, K Devetak, E Deviveiros, PO Dewhurst, A DeWilde, B Dhaliwal, S Dhullipudi, R Di Ciaccio, A Di Ciaccio, L Di Girolamo, A Di Girolamo, B Di Luise, S Di Mattia, A Di Micco, B Di Nardo, R Di Simone, A Di Sipio, R Diaz, MA Diehl, EB Dietrich, J Dietzsch, TA Diglio, S Yagci, KD Dingfelder, J Dinut, F Dionisi, C Dita, P Dita, S Dittus, F Djama, F Djobava, T do Vale, MAB Wemans, AD Doan, TKO Dobbs, M Dobinson, R Dobos, D Dobson, E Dodd, J Doglioni, C Doherty, T Doi, Y Dolejsi, J Dolenc, I Dolezal, Z Dolgoshein, BA Dohmae, T Donadelli, M 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IG Gouighri, M Goujdami, D Goulette, MP Goussiou, AG Goy, C Gozpinar, S Grabowska-Bold, I Grafstrom, P Grahn, KJ Grancagnolo, F Grancagnolo, S Grassi, V Gratchev, V Grau, N Gray, HM Gray, JA Graziani, E Grebenyuk, OG Greenshaw, T Greenwood, ZD Gregersen, K Gregor, IM Grenier, P Griffiths, J Grigalashvili, N Grillo, AA Grinstein, S Gris, P Grishkevich, YV Grivaz, JF Gross, E Grosse-Knetter, J Groth-Jensen, J Gryber, K Guest, D Guicheney, C Guindon, S Gul, U Guler, H Gunther, J Guo, B Guo, J Gutierrez, P Guttman, N Gutzwiller, O Guyot, C Gwenlan, C Gwilliam, CB Haas, A Haas, S Haber, C Hadavand, HK Hadley, DR Haefner, P Hahn, F Haider, S Hajduk, Z Hakobyan, H Hall, D Haller, J Hamacher, K Hamal, P Hamer, M Hamilton, A Hamilton, S Han, L Hanagaki, K Hanawa, K Hance, M Handel, C Hanke, P Hansen, JR Hansen, JB Hansen, JD Hansen, PH Hansson, P Hara, K Hare, GA Harenberg, T Harkusha, S Harper, D Harrington, RD Harris, OM Hartert, J Hartjes, F Haruyama, T Harvey, A Hasegawa, S Hasegawa, Y 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TI Search for high-mass resonances decaying to dilepton final states in pp collisions at root s=7 TeV with the ATLAS detector SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering ID FERMION-PAIR PRODUCTION; GAUGE BOSONS; PARTON DISTRIBUTIONS; E(+)E(-) COLLISIONS; SYMMETRY-BREAKING; EXTRA DIMENSIONS; STANDARD MODEL; LHC; PHYSICS; LEP AB The ATLAS detector at the Large Hadron Collider is used to search for high-mass resonances decaying to an electron-positron pair or a muon-antimuon pair. The search is sensitive to heavy neutral Z' gauge bosons, Randall-Sundrum gravitons, Z* bosons, techni-mesons, Z/gamma bosons, and bosons predicted by Torsion models. Results are presented based on an analysis of pp collisions at a center-of-mass energy of 7 TeV corresponding to an integrated luminosity of 4.9 fb(-1) in the e(+)e(-) channel and 5.0 fb(-1) in the mu(+)mu(-) channel. A Z' boson with Standard Model-like couplings is excluded at 95% confidence level for masses below 2.22 TeV. A Randall-Sundrum graviton with coupling k root M-P1 = 0.1 is excluded at 95% confidence level for masses below 2.16 Tev. Limits on the other models are also presented, including Technicolor and Minimal Z' Models. C1 [Aad, G.; Ahles, F.; Barber, T.; Bernhard, R.; Boehler, M.; Bruneliere, R.; Christov, A.; Consorti, V.; Fehling-Kaschek, M.; Flechl, M.; Glatzer, J.; Hartert, J.; Herten, G.; Horner, S.; Jakobs, K.; Janus, M.; Kononov, A. I.; Kuehn, S.; Lai, S.; Landgraf, U.; Lohwasser, K.; Ludwig, I.; Ludwig, J.; Lumb, D.; Mahboubi, K.; Mohr, W.; Nilsen, H.; Parzefall, U.; Rammensee, M.; Rave, T. C.; Rurikova, Z.; Schmidt, E.; Schumacher, M.; Siegert, F.; Stoerig, K.; Sundermann, J. E.; Temming, K. K.; Thoma, S.; Tsiskaridze, V.; Venturi, M.; Vivarelli, I.; von Radziewski, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Wiik-Fuchs, L. A. 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J.; Beddall, A.; Bingul, A.] Gaziantep Univ, Dept Engn Phys, Gaziantep, Turkey. Istanbul Tech Univ, Dept Phys, TR-80626 Istanbul, Turkey. [Bellagamba, L.; Bertin, A.; Bindi, M.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; Caforio, D.; Ciocca, C.; Corradi, M.; De Castro, S.; Di Sipio, R.; Fabbri, L.; Franchini, M.; Giacobbe, B.; Giusti, P.; Grafstrom, P.; Jha, M. K.; Massa, I.; Mengarelli, A.; Monzani, S.; Negrini, M.; Piccinini, M.; Polini, A.; Rinaldi, L.; Romano, M.; Sbarra, C.; Sbrizzi, A.; Semprirti-Cesari, N.; Spighi, R.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Ist Nazl Fis Nucl, Sez Bologna, Bologna, Italy. [Bertin, A.; Bindi, M.; Caforio, D.; Ciocca, C.; De Castro, S.; Di Sipio, R.; Fabbri, L.; Franchini, M.; Grafstrom, P.; Massa, I.; Mengarelli, A.; Monzani, S.; Piccinini, M.; Romano, M.; Sbrizzi, A.; Semprirti-Cesari, N.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, Dipartimento Fis, Bologna, Italy. [Abajyan, T.; Arutinov, D.; Backhaus, M.; Barbero, M.; Bechtle, P.; Brock, I.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Gaycken, G.; Geich-Gimbel, Ch; Gonella, L.; Haefner, P.; Havranek, M.; Hellmich, D.; Hillert, S.; Huegging, F.; Ince, T.; Karagounis, M.; Khoriauli, G.; Koevesarki, P.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lapoire, C.; Lehmacher, M.; Leyko, A. M.; Limbach, C.; Loddenkoetter, T.; Mayne, A.; Mazur, M.; Moeser, N.; Mueller, K.; Nanava, G.; Nattermann, T.; Nuncio-Quiroz, A. -E.; Pohl, D.; Psoroulas, S.; Schaepe, S.; Schmieden, K.; Schmitz, M.; Schultens, M. J.; Schwindt, T.; Stillings, J. A.; Therhaag, J.; Tsung, J. -W.; Uchida, K.; Uhlenbrock, M.; Urquijo, P.; Vogel, A.; von Toerne, E.; Wang, T.; Wermes, N.; Wiernemann, P.; Zendler, C.; Zimmermann, R.; Zimmermann, S.] Univ Bonn, Inst Phys, Bonn, Germany. [Ahlen, S. P.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Shank, J. 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D.; Klimentov, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Majewski, S.; Metcalfe, J.; Nevski, P.; Okawa, H.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Park, W.; Pleier, M. -A.; Poblaguev, A.; Polychronakos, V.; Pravahan, R.; Protopopescu, S.; Purohit, M.; Rahm, D.; Rajagopalan, S.; Redlinger, G.; Sawyer, L.; Sircar, A.; Snyder, S.; Steinberg, P.; Stumer, I.; Takai, H.; Tamsett, M. C.; Triplett, N.; Undrus, A.; Wenaus, T.; Ye, S.; Yu, D.; Zaytsev, A.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Badescu, E.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Cuciuc, C. -M.; Dinut, F.; Dita, P.; Dita, S.; Micu, L.; Olariu, A.; Pantea, D.; Popeneciu, G. A.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Darlea, G. L.] Univ Politehn Bucuresti, Bucharest, Romania. W Univ Timisoara, Timisoara, Romania. [Gonzalez Silva, M. L.; Otero y Garzon, G.; Piegaia, R.; Romeo, G.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Ask, S.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Buttinger, W.; Carter, J. R.; Chapman, J. D.; Cowden, C.; French, S. T.; Frost, J. A.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Moeller, V.; Parker, M. A.; Robinson, D.; Sandoval, T.; Thomson, M.; Ward, C. P.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Gillberg, D.; Koffas, T.; Liu, C.; Marchand, J. F.; McCarthy, T. G.; Oakham, F. G.; Randrianarivony, K.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Anastopoulos, C.; Anghinolfi, F.; Baak, M. A.; Bachas, K.; Banfi, D.; Battistin, M.; Bellina, F.; Bellomo, M.; Beltramello, O.; Berge, D.; Bianchi, R. M.; Blanchot, G.; Bogaerts, J. A.; Boyd, J.; Bremer, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Catmore, J. R.; Cattai, A.; Cerri, A.; Barajas, C. A. 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J.; Boveia, A.; Canelli, F.; Choudalakis, G.; Fiascaris, M.; Gardner, R. W.; Plante, I. Jen-La; Kapliy, A.; Melachrinos, C.; Merritt, F. S.; Meyer, C.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Shochet, M. J.; Tompkins, L.; Tuggle, J. M.; Vukotic, I.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Diaz, M. A.; Pino, S. A. Olivares; Quinonez, F.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Carquin, E.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.] Univ Tecn Feder Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Jin, S.; Lu, F.; Ouyang, Q.; Ruan, X.; Shan, L. Y.; Yao, L.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Han, L.; Jiang, Y.; Li, S.; Liu, M.; Liu, Y.; Peng, H.; Wang, H.; Wu, Y.; Xu, C.; Zhang, D.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Feng, C.; Ge, P.; Meng, Z.; Miao, J.; Zhan, Z.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Toro, R. Camacho; Cinca, D.; Donini, J.; Febbraro, R.; Ghodbane, N.; Gris, Ph; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Vazeille, F.] Clermont Univ, Phys Corpusculaire Lab, Aubiere, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Toro, R. Camacho; Cinca, D.; Donini, J.; Febbraro, R.; Ghodbane, N.; Gris, Ph; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Vazeille, F.] Univ Clermont Ferrand, Aubiere, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Toro, R. Camacho; Cinca, D.; Donini, J.; Febbraro, R.; Ghodbane, N.; Gris, Ph; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Vazeille, F.] CNRS IN2P3, Aubiere, France. [Altheimer, A. 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[Capua, M.; Crosetti, G.; Fazio, S.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Morello, G.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Banas, E.; Blocki, J.; de Renstrom, P. A. Bruckman; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa; Malecki, P.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Turala, M.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.; Zemla, A.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Yagci, K. Dindar; Firan, A.; Hadavand, H. K.; Hoffman, J.; Ishmukhametov, R.; Joffe, D.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Rios, R. R.; Sekula, S. J.; Stroynowski, R.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Ahsan, M.; Izen, J. M.; Lou, X.; Reeves, K.; Wong, W. C.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Kuutmann, E. Bergeaas; Bloch, I.; Dassoulas, J. A.; Dietrich, J.; Ehrenfeld, W.; Ferrara, V.; Fischer, G.; Friedrich, C.; Glazov, A.; Goebel, M.; Fajardo, L. S. Gomez; Da Costa, J. Gonca Lves Pinto Firmino; Gosdzik, B.; Grahn, K-J.; Gregor, I. M.; Hiller, K. H.; Huettmann, A.; Husemann, U.; Belenguer, M. Jimenez; Johnert, S.; Karnevskiy, M.; Katzy, J.; Kono, T.; Kuhl, T.; Lange, C.; Lobodzinska, E.; Ludwig, D.; Medinnis, M.; Moenig, K.; Naumann, T.; Cavalcanti, T. Perez; Petschull, D.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Zhu, H.] DESY, D-2000 Hamburg, Germany. [Bunse, M.; Esch, H.; Goessling, C.; Hirsch, F.; Jung, C. A.; Klingenberg, R.; Reisinger, I.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Czodrowski, P.; Friedrich, F.; Goepfert, T.; Kobel, M.; Leonhardt, K.; Ludwig, A.; Nader, W. F.; Morgenstern, M.; Prudent, X.; Rudolph, C.; Schnoor, U.; Schwierz, R.; Seifert, F.; Steinbach, P.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Ko, B. R.; Kotwal, A.; Oh, S. H.; Wang, C.; Yamaoka, J.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Buckley, A. G.; Clark, P. J.; Debenedetti, C.; Harrington, R. D.; Martin, V. J.; O'Brien, B. J.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Cerutti, F.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.; Volpi, G.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Abdelalim, A. A.; Alexandre, G.; Backes, M.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; Blondel, A.; Bucci, F.; Clark, A.; Dao, V.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Iacobucci, G.; La Rosa, A.; Lister, A.; Latour, B. Martin dit; Mermod, P.; Herrera, C. Mora; Nektarijevic, S.; Nikolics, K.; Pasztor, G.; Picazio, A.; Pohl, M.; Rosbach, K.; Rosselet, L.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Beccherle, R.; Caso, C.; Dameri, M.; Darbo, G.; Ferretto Parodi, A.; Gagiardi, G.; Gemme, C.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Genoa, Italy. [Barberis, D.; Caso, C.; Dameri, M.; Ferretto Parodi, A.; Gagiardi, G.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Chikovani, L.; Tskiadadze, E. G.] Tbilisi State Univ, E Andronikashvili Inst Phys, GE-380086 Tbilisi, Rep of Georgia. [Djobava, T.; Khubua, J.; Mchedlidze, G.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, GE-380086 Tbilisi, Rep of Georgia. [Dueren, M.; Stenzel, H.] Univ Giessen, Inst Phys 2, D-6300 Giessen, Germany. [Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Bussey, P.; Buttar, C. M.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Edwards, N. C.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Kar, D.; Kenyon, M.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Robson, A.; Saxon, D. H.; Smith, K. M.; St Denis, R. F.; Steele, G.; Thompson, A. S.; Wraight, K.; Wright, M.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bierwagen, K.; Blumenschein, U.; Brandt, O.; Erdmann, J.; Evangelakou, D.; George, M.; Grosse-Knetter, J.; Guindon, S.; Haller, J.; Hamer, M.; Henrichs, A.; Hensel, C.; Keil, M.; Knue, A.; Kohn, F.; Krieger, N.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Mann, A.; Meyer, J.; Morel, J.; Pashapour, S.; Quadt, A.; Roe, A.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Uhrmacher, M.; Schroeder, T. Vazquez; Weber, P.; Weingarten, J.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Stark, J.; Sun, X.; Trocme, B.; Wang, J.; Weydert, C.] Univ Grenoble 1, Lab Phys Subatom & Cosmol, Grenoble, France. [Albrand, S.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Stark, J.; Sun, X.; Trocme, B.; Wang, J.; Weydert, C.] CNRS IN2P3, Grenoble, France. [Albrand, S.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Stark, J.; Sun, X.; Trocme, B.; Wang, J.; Weydert, C.] Inst Natl Polytech Grenoble, F-38031 Grenoble, France. [Addy, T. N.; Harvey, A.; McFarlane, K. W.; Shin, T.; Vassiakopoulos, V. I.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Belloni, A.; Catastini, P.; Conti, G.; Huth, J.; Jeanty, L.; Kagan, M.; Mateos, D. Lopez; Outschoorn, V. Martinez; Mercurio, K. M.; Mills, C.; Morii, M.; Skottowe, H. P.; Smith, B. C.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Anders, G.; Andrei, V.; Davygora, Y.; Dietzsch, T. A.; Geweniger, C.; Hanke, P.; Henke, M.; Khomich, A.; Kluge, E. -E.; Lang, V. S.; Endermann, V.; Lepold, F.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, D-6900 Heidelberg, Germany. [Kugel, A.; Maenner, R.; Schroer, N.] Heidelberg Univ, ZITI Inst Tech Informat, D-6800 Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Cwetanski, P.; Gagnon, P.; Jain, V.; Luehring, F.; Ogren, H.; Pewell, J.; Poveda, J.; Price, D.; Whittington, D.; Yang, Y.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Epp, B.; Jussel, P.; Kneringer, E.; Kuhn, D.; Lukas, W.; Rudolph, G.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Limper, M.; Mallik, U.; Pylypchenko, Y.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Rosenberg, E. I.; Ruiz-Martinez, A.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Aleksandrov, I. N.; Bardin, D. Y.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Grigalashvili, N.; Huseynov, N.; Kalinovskaya, L. V.; Kazarinov, M. Y.; Kekelidze, G. D.; Kharchenko, D.; Khramov, E.; Kolesnikov, V.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Maleev, V. P.; Mayne, A.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Pozdnyakov, V.; Rumyantsev, L.; Rusakovich, N. A.; Sadykov, R.; Shiyakova, M.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.; Zimin, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Arai, Y.; Doi, Y.; Haruyama, T.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Makida, Y.; Manabe, A.; Mitsui, S.; Nagano, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Havakawa, T.; King, M.; Kishimoto, T.; Kitamura, T.; Kurashige, H.; Matsushita, T.; Ochi, A.; Suzuki, Y.; Takeda, H.; Tani, K.; Watanabe, I.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Sasao, N.; Sumida, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Davidson, R.; de Mora, L.; Dearnaley, W. J.; Fox, H.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Bianco, M.; Cataldi, G.; Chiodini, G.; Gorini, E.; Grancagnolo, F.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, Lecce, Italy. [Bianco, M.; Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Piece, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Greenshaw, T.; Gwilliam, C. B.; Hayward, H. S.; Jackson, J. N.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kluge, T.; Kretzschmar, J.; Laycock, P.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Sellers, G.; Vossebeld, J. H.; Waller, P.; Wrona, B.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Dolenc, I.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Dolenc, I.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Adragna, P.; Bona, M.; Carter, A. A.; Cerrito, L.; Eisenhandlerm, E.; Ellis, K.; Goddard, J. R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Poll, J.; Rizvi, E.; Salamanna, G.; Castanheira, M. Teixeira Dias; Wiglesworth, C.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Alam, M. A.; Berry, T.; Boisvert, V.; Brooks, T.; Cantrill, R.; Cowan, G.; Duguid, L.; Edwardsm, C. A.; George, S.; Goncalo, R.; Hayden, D.; Pastore, Fr; Rose, M.; Spano, F.; Strong, J. A.; Teixeiro-Dias, P.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Baker, S.; Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Chislett, R. T.; Christidi, I. A.; Cooper, B. D.; Davison, A. R.; Dobson, E.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Larabourne, L.; Monk, J.; Nash, M.; Nurse, E.; Prabhu, R.; Sherwood, P.; Simmons, B.; Taylor, C.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Cavalleri, P.; Chareyre, E.; Davignon, O.; De Cecco, S.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph; Theveneaux-Pelzer, T.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Cavalleri, P.; Chareyre, E.; Davignon, O.; De Cecco, S.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph; Theveneaux-Pelzer, T.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Cavalleri, P.; Chareyre, E.; Davignon, O.; De Cecco, S.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph; Theveneaux-Pelzer, T.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] CNRS IN2P3, Paris, France. [Akesson, T. P. A.; Alonso, A.; Bocchetta, S. S.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Jarlskog, G.; Lundberg, B.; Lytken, E.; Meirose, B.; Mjornmark, J. U.; Smirnova, O.] Lund Univ, Inst Fys, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Labarga, L.; Llorente Merino, J.; March, L.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Aharrouche, M.; Arnaez, O.; Blum, W.; Buescher, V.; Caputo, R.; Eckweiler, S.; Edmonds, K.; Ellinghaus, F.; Ertel, E.; Fiedler, F.; Fleckner, J.; Goeringer, C.; Handel, C.; Hohlfeld, M.; Hsu, P. J.; Jia, W.; Kawamura, G.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lungwitz, M.; Maettig, S.; Masetti, L.; Meyer, C.; Moreno, D.; Mueller, T.; Neusiedl, A.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schroeder, C.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.] Johannes Gutenberg Univ Mainz, Inst Phys, D-6500 Mainz, Germany. [Almond, J.; Borri, M.; Brown, G.; Chavda, V.; Cox, B. E.; Da Via, C.; Duerdoth, I. P.; Forti, A.; Howarth, J.; Ibbotson, M.; Joshi, K. D.; Klinger, J. A.; Lane, J. L.; Loebinger, F. K.; Marx, M.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Pilkington, A. D.; Robinson, J. E. M.; Schwanenberger, C.; Snow, S. W.; Watts, S.; Woudstra, M. J.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aoun, S.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Li, S.; Maurer, J.; Monnier, E.; Odier, J.; Pralavorio, P.; Rozanov, A.; Talby, M.; Tannoury, N.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aoun, S.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Li, S.; Maurer, J.; Monnier, E.; Odier, J.; Pralavorio, P.; Rozanov, A.; Talby, M.; Tannoury, N.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] CNRS IN2P3, Marseille, France. [Brau, B.; Colon, G.; Dallapiccola, C.; Mcade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Caron, B.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Dobbs, M.; Dufour, M-A.; Guler, H.; Klemetti, M.; Mc Donald, J.; Robertson, S. H.; Rios, C. Santamarina; Schram, M.; Stockton, M. C.; Vachon, B.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Davidson, N.; Diglio, S.; Jennens, D.; Kubota, T.; Limosani, A.; Moorhead, G. F.; Hanninger, G. Nunes; Phan, A.; Shao, Q. T.; Taylor, G. N.; Thong, W. M.; Volpi, M.; White, M. J.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Armbruster, A. J.; Borroni, S.; Chapman, J. W.; Cirilli, M.; Dai, T.; Diehl, E. B.; Ferretti, C.; Goldfarb, S.; Harper, D.; Levin, D.; Li, X.; Liu, H.; Liu, J. B.; Liu, L.; Mc Kee, S. P.; Neal, H. A.; Panikashvili, N.; Purdham, J.; Qian, J.; Scheirich, D.; Thun, R. P.; Walch, S.; Wilson, A.; Wooden, G.; Wu, Y.; Yang, H.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Fedorko, W.; Hauser, R.; Heim, S.; Holzbauer, J. L.; Huston, J.; Koll, J.; Linnemann, J. T.; Mangeard, P. S.; Martin, B.; Miller, R. J.; Pope, B. G.; Schwienhorst, R.; Stelzer, H. J.; Tollefson, K.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alessandria, F.; Alimonti, G.; Andreazza, A.; Baccaglioni, G.; Besana, M. I.; Broggi, F.; Carminati, L.; Cavalli, D.; Citterio, M.; Consonni, S. M.; Costa, G.; Fanti, M.; Favareto, A.; Giugni, D.; Koletsou, I.; Lari, T.; Mandelli, L.; Mazzanti, M.; Meloni, F.; Merola, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Rivoltella, G.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Vegni, G.; Vopini, G.] Ist Nazl Fis Nucl, Sez Milano, Milan, Italy. [Andreazza, A.; Besana, M. I.; Carminati, L.; Consonni, S. M.; Fanti, M.; Favareto, A.; Meloni, F.; Perini, L.; Pizio, C.; Ragusa, F.; Rivoltella, G.; Simoniello, R.; Turra, R.; Vegni, G.] Univ Milan, Dipartimento Fis, Milan, Italy. [Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Satsounkevitch, I.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus. [Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Azuelos, G.; Banerjee, P.; Bouchami, J.; Davies, M.; Giunta, M.; Guler, H.; Leroy, C.; Martin, J. P.; Mehdiyev, R.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu; Shmeleva, A.; Snesarev, A. A.; Tikhomirov, V. O.] Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Romaniouk, A.; Shulga, F.; Smirnov, S. Yu; Smirnov, Y.; Soldatov, E. Yu; Timoshenko, S.] Moscow Engn & Phys Inst MEPhI, Moscow, Russia. [Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Rud, V. I.; Sivoklokov, S. Yu; Smirnova, L. N.; Sulin, V. V.] Moscow MV Lomonosov State Univ, Skobellsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Beale, S.; Becker, S.; Biebel, O.; Calfayan, P.; de Graat, J.; Duckeck, G.; Ebke, J.; Elmsheuser, J.; Eng, A.; Galea, C.; Heller, C.; Hertenberger, R.; Kummer, C.; Legger, F.; Lichtnecker, M.; Lorenz, J.; Mameghani, R.; Mueller, T. A.; Nunnemann, T.; Oakes, L. B.; Rauscher, F.; Reznicek, P.; Sanders, M. P.; Schaile, D.; Schieck, J.; Serfon, C.; Staude, A.; Vladoiu, D.; Walker, R.; Will, J. Z.; Zhou, B.; Zhuang, X.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Beimforde, M.; Bethke, S.; Bittner, B.; Bronner, J.; Capriotti, D.; Cortiana, G.; Dubbert, J.; Flowerdew, M. J.; Giovannini, P.; Jantsch, A.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kotov, S.; Kroha, H.; Macchiolo, A.; Manfredini, A.; Mayne, A.; Menke, S.; Moser, H. G.; Nagel, M.; Nisius, R.; Oberlack, H.; Pahl, C.; Pospelov, G. E.; Potrap, I. N.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph; Seuster, R.; Stern, S.; Stonjek, S.; Vanadia, M.; von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.; Zhuravlov, V.] Max Planck Inst Phys Werner Heisenberg Inst, Munich, Germany. [Gan, K. K.; Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Shimizu, S.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Shimizu, S.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Capasso, L.; Carlino, G.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; della Volpe, D.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Musto, E.; Patricelli, S.; Sanchez, A.; Sekhniaidze, G.] Ist Nazl Fis Nucl, Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Capasso, L.; Chiefari, G.; della Volpe, D.; Giordano, R.; Merola, L.; Musto, E.; Patricelli, S.; Sanchez, A.] Univ Naples Federico II, Dipartimento Sci Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Chelstowska, M. A.; De Groot, N.; Filthaut, F.; Klok, P. F.; Koenig, A. C.; Koetsveld, F.; Raas, M.; Salvucci, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Doxiadis, A. D.; Ferrari, P.; Garitaonandia, H.; Geerts, D. A. A.; Gosselink, M.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kayl, M. S.; Klous, S.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Luickx, G.; Massaro, G.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Pani, P.; Rijpstra, M.; Ruckstuhl, N.; Ta, D.; Tsiakiris, M.; Turlay, E.; Van der Deij, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van der Poel, E.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.] Nikhef Natl Inst Subatom Phys, Amsterdam, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Doxiadis, A. D.; Ferrari, P.; Garitaonandia, H.; Geerts, D. A. A.; Gosselink, M.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kayl, M. S.; Klous, S.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Luickx, G.; Massaro, G.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Pani, P.; Rijpstra, M.; Ruckstuhl, N.; Ta, D.; Tsiakiris, M.; Turlay, E.; Van der Deij, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuw, R.; van der Poel, E.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.] Univ Amsterdam, Amsterdam, Netherlands. [Calkins, R.; Chakraborty, D.; Cole, S.; de Lima, J. G. Rocha; Suhr, C.; Yurkewicz, A.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A.; Beloborodova, O.; Bobrovnikov, V. B.; Bogdanchikov, A.; Kazanin, V. A.; Kolachev, G. M.; Korol, A.; Malyshev, V.; Maslennikov, A. L.; Orlov, I.; Peleganchuk, S. V.; Schamov, A. G.; Skovpen, K.; Soukharev, A.; Talyshev, A.; Tikhonov, Y. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Budick, B.; Casadei, D.; Cranmer, K.; van Huysduynen, L. Hooft; Kaplan, B.; Konoplich, R.; Krasznahorkay, A.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.; Prokofiev, K.; Shibata, A.; Zhao, L.] NYU, Dept Phys, New York, NY 10003 USA. [Fisher, M. J.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Rahimi, A. M.; Strang, M.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Gutierrez, P.; Jana, D. K.; Marzin, A.; Meera-Lebbai, R.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Snow, J.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Khanov, A.; Rizatdinova, F.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Hamal, P.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Potter, C. T.; Ptacek, E.; Radloff, P.; Reinsch, A.; Searey, J.; Sinev, N. B.; Strom, D. M.; Torrence, E.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Andari, N.; Arnault, C.; Auge, E.; Barrillon, P.; Benoit, M.; Binet, S.; Bourdarios, C.; De la Taille, C.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Henrot-Versille, S.; Hrivnac, J.; Iconoraidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Matricon, P.; Niedercorn, F.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Ruan, X.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Serin, L.; Shamim, M.; Simion, S.; Tanaka, R.; Teinturier, M.; Veillet, J. J.; Wicek, F.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Andari, N.; Arnault, C.; Auge, E.; Barrillon, P.; Benoit, M.; Binet, S.; Bourdarios, C.; De la Taille, C.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Henrot-Versille, S.; Hrivnac, J.; Iconoraidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Matricon, P.; Niedercorn, F.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Ruan, X.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Serin, L.; Shamim, M.; Simion, S.; Tanaka, R.; Teinturier, M.; Veillet, J. J.; Wicek, F.; Zerwas, D.; Zhang, Z.] CNRS IN2P3, Orsay, France. [Hanagaki, K.; Hirose, M.; Lee, J. S. H.; Meguro, T.; Nomachi, M.; Sugaya, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Buran, T.; Cameron, D.; Gjelsten, B. K.; Lund, E.; Ould-Saada, F.; Pajchel, K.; Read, A. L.; Rohne, O.; Samset, B. H.; Smestad, S. L.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Apolle, R.; Barr, A. J.; Boddy, C. R.; Brandt, G.; Buchanan, J.; Buckingham, R. M.; Coniavitis, E.; Cooper-Sarkar, A. M.; Dafinca, A.; Davies, E.; Gallas, E. J.; Gwenlan, C.; Hall, D.; Hays, C. P.; Howard, J.; Huffman, T. B.; Issever, C.; King, R. S. B.; Kogan, L. A.; Korn, A.; Larner, A.; Lewis, A.; Liang, Z.; Livermore, S. S. A.; Mattravers, C.; Mayne, A.; Nickerson, R. B.; Pinder, A.; Robichaud-Veronneau, A.; Ryder, N. C.; Short, D.; Tseng, J. C-L.; Vickey, T.; Viehhauser, G. H. A.; Weidberg, A. R.; Whitehead, S. R.; Young, C. J.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Colombo, T.; Conta, C.; Ferrari, R.; Franchino, S.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Uslenghi, M.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, Pavia, Italy. [Colombo, T.; Conta, C.; Franchino, S.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.; Uslenghi, M.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Alison, J.; Brendlinger, K.; Degenhardt, J.; Fratina, S.; Hines, E.; Hong, T. M.; Jackson, B.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Olivito, D.; Ospanov, R.; Reece, R.; Saxon, J.; Schaefer, D.; Stahlman, J.; Thomson, E.; Wagner, P.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Bertolucci, F.; Cascella, M.; Cavasinni, V.; Crescioli, F.; Del Prete, T.; Dotti, A.; Roda, C.; Sarri, F.; White, S.; Zinonos, Z.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Bertolucci, F.; Cascella, M.; Cavasinni, V.; Crescioli, F.; Del Prete, T.; Dotti, A.; Roda, C.; Sarri, F.; White, S.; Zinonos, Z.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Boudreau, J.; Cleland, W.; Escobar, C.; Kittelmann, T.; Mueller, J.; Prieur, D.; Savinov, V.; Yoosofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amorim, A.; Anjos, N.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Do Valle Wemans, A.; Fiolhais, M. C. N.; Gomes, A.; Jorge, P. M.; Li, H.; Lin, S. C.; Lopes, L.; Machado Miguens, J.; Maio, A.; Maneira, J.; Oliveira, M.; Onofre, A.; Palma, A.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. [Bohm, J.; Chudoba, J.; Gallus, P.; Gunther, J.; Jakoubek, T.; Juranek, V.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Marcisovsky, M.; Mikestikova, M.; Myska, M.; Nemecek, S.; Ruzicka, P.; Schovancova, J.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Tic, T.; Valenta, J.; Vrba, V.; Zeman, M.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Kodys, P.; Leitner, R.; Novakova, J.; Rybar, M.; Spousta, M.; Strachota, P.; Suk, M.; Sykora, T.; Tas, P.; Valkar, S.; Vorobel, V.; Wilhelm, I.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Augsten, K.; Holy, T.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Kral, V.; Krejci, F.; Pospisil, S.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solar, M.; Solc, J.; Sopko, V.; Sopko, B.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Ammosov, V. V.; Borisov, A.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Ivashin, A. V.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.; Zmouchko, V. V.] Inst High Energy Phys, State Res Ctr, Protvino, Russia. [Adye, T.; Apolle, R.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Gillman, A. R.; Haywood, S. J.; Kirk, J.; Mattravers, C.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Nash, M.; Norton, P. R.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Strube, J.; Tyndel, M.; Wickens, F. J.; Wielers, A.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Benslama, K.; Smit, G. V. Ybeles] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Artoni, G.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Pedis, D.; De Salvo, A.; De Zorzi, G.; Dionisi, C.; Falciano, S.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Potaecorvo, L.; Rescigno, M.; Rosati, S.; Rossi, E.; Tehrani, F. Safai; Sidoti, A.; Camillocci, E. Soltaroli; Vari, R.; Veneziano, S.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma 1, Rome, Italy. [Artoni, G.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Zorzi, G.; Dionisi, C.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Messina, A.; Rossi, E.; Camillocci, E. Soltaroli; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Di Simone, A.; Liberti, B.; Marchese, F.; Mazzaferro, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Cattani, G.; Di Ciaccio, A.; Di Simone, A.; Marchese, F.; Mazzaferro, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Branchini, P.; Ceradini, F.; Di Luise, S.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Stanescu, C.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Luise, S.; Orestano, D.; Pastore, F.; Petrucci, F.] Univ Roma Tre, Dipartimento Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.; Labaka, S.] Reseau Univ Phys Hautes Energies Univ Hassan II, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA Marrakech, Marrakech, Morocco. Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [El Moursli, R. Cherkaoui] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Abreu, H.; Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Bolnet, N. M.; Boonekamp, M.; Chevalier, L.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Gauthier, L.; Giraud, P. F.; Guyot, C.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Legendre, M.; Maiani, C.; Mal, P.; Ramos, J. A. Manjarres; Mansoulie, B.; Meyer, J-P.; Mijovic, L.; Morange, N.; Mountricha, E.; Hong, V. Nguyen Thi; Nicolaidou, R.; Ouraou, A.; Resende, B.; Royon, C. R.; Schune, Ph; Schwindling, J.; Simard, O.; Virchaux, M.; Vranjes, N.; Xiao, M.; Xu, C.] CEA Saclay Commissariat Energie Atom, DSM IRFU, Gif Sur Yvette, France. [Chouridou, S.; Damiani, D. S.; Grillo, A. A.; Hare, G. A.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Mitrevski, J.; Nielsen, J.; Sadrozinski, H. F-W; Schumm, B. A.; Seiden, A.; Stekl, I.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Beckingham, M.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Keller, J. S.; Lubatti, H. J.; Rompotis, N.; Rothberg, J.; Verducci, M.; Watts, G.; Zhao, T.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Duxfield, R.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Koroolkova, E. V.; Mayne, A.; Mcfayden, J. A.; Miyagawa, P. S.; Owen, S.; Paganis, Li.; Suruliz, K.; Tovey, D. R.; Tsionou, D.; Tua, A.; Xu, D.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Gryber, K.; Holder, M.; Ibragimov, I.; Rammes, M.; Rosentthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-5900 Siegen, Germany. [Dawe, E.; Godfrey, J.; Kvita, J.; O'Neill, D. C.; Petteni, M.; Stelzer, B.; Tanasijczuk, A. J.; Trottier-McDonald, M.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Butler, B.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Grenier, P.; Haas, A.; Hansson, P.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nelson, T. K.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Smith, D.; Strauss, E.; Su, D.; Wilson, M. G.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Batkova, L.; Blazek, T.; Federic, P.; Pecsy, M.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Fernando, W.; Kladiva, E.; Seman, M.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Aurousseau, M.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Hamilton, A.; Leney, K. J. C.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Asman, B.; Bendtz, K.; Bohm, C.; Clement, C.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Holmgren, S. O.; Johansen, M.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Papadelis, A.; Sellden, B.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Stockholm Univ, Dept Phys, Stockholm, Sweden. [Asman, B.; Bendtz, K.; Clement, C.; Gellerstedt, K.; Hellman, S.; Johansen, M.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Sjolin, J.; Strandberg, S.; Tylmad, M.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Ahmad, A.; Arfaoui, S.; Devetak, E.; DeWilde, B.; Engelmann, R.; Farley, J.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Ahmad, A.; Arfaoui, S.; Devetak, E.; DeWilde, B.; Engelmann, R.; Farley, J.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Bartsch, V.; De Santo, A.; Martin-Haugh, S.; Potter, C. J.; Rose, A.; Salvatore, F.; Sutton, M. R.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Bangert, A.; Cuthbert, C.; Patel, N.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Waugh, A. T.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Chu, M. L.; Hou, S.; Lee, S. C.; Lin, S. C.; Liu, D.; Mazini, R.; Meng, Z.; Ren, Z. L.; Soh, D. A.; Teng, P. K.; Wang, J.; Wang, S. M.; Weng, Z.; Zhou, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Harpaz, S. Behar; Kajomovitz, E.; Rozen, Y.; Tarem, S.; Vallecorsa, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Bella, G.; Benary, O.; Benhammou, Y.; Etzion, E.; Gershon, A.; Ginzburg, J.; Guttman, N.; Hod, N.; Munwes, Y.; Oren, Y.; Reinherz-Aronis, E.; Sadeh, I.; Silveri, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Iliadis, D.; Kordas, K.; Kouskoura, V.; Nomidis, I.; Petridis, A.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, K.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yamazaki, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, K.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yamazaki, T.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Ishitsuka, M.; Jinnouchi, O.; Kanno, T.; Kuze, M.; Nagai, R.; Nobe, T.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Bailey, D. C.; Bain, T.; Brelier, B.; Cheung, S. L.; Dhaliwal, S.; Farooque, T.; Fatholahzadeh, B.; Gibson, A.; Guo, B.; Ilic, N.; Keung, J.; Knecht, N. S.; Krieger, P.; Martens, F. K.; Orr, R. S.; Rezvani, R.; Savard, P.; Sinervo, P.; Spreitzer, T.; Tardif, D.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Fortin, D.; Gingrich, D. M.; Koutsman, A.; Losty, M. J.; Nugent, I. M.; Oakham, F. G.; Oram, C. J.; Codina, F. Perez; Savard, P.; Schouten, D.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Canepa, A.; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hanawa, K.; Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Kurata, M.; Nagai, K.; Ukegawa, F.] Univ Tsukuba, Inst Pure & Appl Sci, Tsukuba, Ibaraki 3058571, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Napier, A.; Rolli, S.; Sliwa, K.; Todorova-Nova, S.; Wetter, J.] Tufts Univ, Ctr Sci & Technol, Medford, MA 02155 USA. [Losada, M.; Loureiro, K. F.; Navas, L. Mendoza; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Avolio, G.; Deng, J.; Farrell, S.; Eschrich, I. Gough; Lankford, A. J.; Magnoni, L.; Mete, A. S.; Nelson, A.; Scannicchio, D. A.; Schernau, M.; Taffard, A.; Toggerson, B.; Unel, G.; Werth, M.; Wheeler-Ellis, S. J.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Del Papa, C.; Pinamonti, M.; Shaw, K.; Soualah, R.] Ist Nazl Fis Nucl, Grp Collegato Udine, Udine, Italy. [Acharya, B. S.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Del Papa, C.; Giordani, M. P.; Pinamonti, M.; Shaw, K.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Coggeshall, J.; Cortes-Gonzalez, A.; Errede, D.; Errede, S.; Lie, K.; Liss, T. M.; McCarn, A.; Neubauer, M. S.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Brenner, R.; Buszello, C. P.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Pelikan, D.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Maleev, V. P.; Marti-Garcia, S.; Minano Moya, M.; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] CSIC, Valencia, Spain. [Axen, D.; Gay, C.; Gecse, Z.; Loh, C. W.; Mills, W. J.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Astbury, A.; Bansal, V.; Berghaus, F.; Courneyea, L.; Fincke-Keeler, M.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Lessard, J-R.; Marino, C. P.; Martyniuk, A. C.; McPherson, R. A.; Ouellette, E. A.; Plamondon, M.; Sobie, R.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Farrington, S. M.; Jones, G.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Kimura, N.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Alon, R.; Barak, L.; Bressler, S.; Duchovni, F.; Frank, T.; Gabizon, O.; Gross, E.; Groth-Jensen, J.; Klier, A.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Milstein, D.; Roth, I.; Silbert, O.; Smakhtin, V.; Vitells, O.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Asfandiyarov, R.; Banerjee, Sw; Montoya, G. D. Carrillo; Hernandez, A. M. Castaneda; Castaneda-Miranda, E.; Chen, X.; Di Mattia, A.; Dos Anjos, A.; Fang, Y.; Catillo, L. R. Flores; Gutzwiller, O.; Ji, H.; Ju, X.; Kashif, L.; Li, H.; Ma, L. L.; Garcia, B. R. Mellado; Ming, Y.; Pan, Y. B.; Morales, M. I. Pedraza; Quayle, W. B.; Sarangi, T.; Wang, H.; Wiedenmann, W.; Wu, S. L.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Fleischmann, P.; Meyer, J.; Redelbach, A.; Siragusa, G.; Stroehmer, R.; Trefzger, T.] Univ Wurzburg, Fak Phys & Astron, Wurzburg, Germany. [Barisonzi, M.; Becker, A. K.; Becks, K. H.; Boek, J.; Braun, H. M.; Cornelissen, T.; Duda, D.; Fleischmann, S.; Flick, T.; Gerlach, P.; Glitza, K. W.; Gorfine, G.; Hamacher, K.; Harenberg, T.; Henss, T.; Hirschbuehl, D.; Kalinin, S.; Kersten, S.; Khoroshilov, A.; Kohlmann, S.; Lantzsch, K.; Lenzen, G.; Maettig, P.; Mechtel, M.; Neumann, M.; Pataraia, S.; Sandhoff, M.; Sartisohn, G.; Schultes, J.; Sturm, P.; Voss, T. T.; Wagner, W.; Wahlen, H.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany. [Adelman, J.; Baker, O. K.; Bedikian, S.; Almenar, C. Cuenca; Czyczula, Z.; Demers, S.; Garberson, F.; Golling, T.; Guest, D.; Lagouri, T.; Lee, L.; Loginov, A.; Sherman, D.; Tipton, P.; Wall, R.; Walsh, B.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Biscarat, C.; Cogneras, E.; Rahal, G.] Ctr Calcul CNRS IN2P3, Villeurbanne, France. [Amorim, A.; Maio, A.; Pina, J.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amorim, A.; Maio, A.; Pina, J.] Univ Lisbon, CFNUL, Lisbon, Portugal. [Bawa, H. S.; Lowe, A. J.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beloborodova, O.; Talyshev, A.; Tikhonov, Y. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Canelli, F.] Fermilab Natl Accelerator Lab, Batavia, IL USA. [Carvalho, J.; Fiolhais, M. C. N.; Oliveira, M.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Hernandez, A. M. Castaneda] UASLP, Dept Phys, San Luis Potosi, Mexico. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Demirkoz, B.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Dhullipudi, R.; Greenwood, Z. D.; Sawyer, L.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Do Valle Wemans, A.] Univ Nova Lisboa, Dep Fis, Caparica, Portugal. [Do Valle Wemans, A.] Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, Caparica, Portugal. [Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Wildt, M. A.] Univ Hamburg, Inst Expt Phys, Hamburg, Germany. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Liang, Z.; Soh, D. A.; Weng, Z.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou, Peoples R China. Acad Sinica, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Nessi, M.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Park, W.; Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Pasztor, G.; Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Perez, K.] CALTECH, Pasadena, CA 91125 USA. [Richter-Was, E.] Jagiellonian Univ, Inst Phys, Krakow, Poland. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. RP Aad, G (reprint author), Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. EM atlas.publications@cern.ch RI Petrucci, Fabrizio/G-8348-2012; Annovi, Alberto/G-6028-2012; Alexa, Calin/F-6345-2010; Gutierrez, Phillip/C-1161-2011; Wemans, Andre/A-6738-2012; Fazio, Salvatore /G-5156-2010; Bergeaas Kuutmann, Elin/A-5204-2013; Cascella, Michele/B-6156-2013; messina, andrea/C-2753-2013; Weigell, Philipp/I-9356-2012; de Groot, Nicolo/A-2675-2009; Moorhead, Gareth/B-6634-2009; Ma, Hong/F-2725-2011; Fassi, Farida/F-3571-2016; la rotonda, laura/B-4028-2016; Karyukhin, Andrey/J-3904-2014; Capua, Marcella/A-8549-2015; Tartarelli, Giuseppe Francesco/A-5629-2016; Maneira, Jose/D-8486-2011; KHODINOV, ALEKSANDR/D-6269-2015; Goncalo, Ricardo/M-3153-2016; Gauzzi, Paolo/D-2615-2009; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Martinez, Mario /I-3549-2015; Monzani, Simone/D-6328-2017; Grancagnolo, Francesco/K-2857-2015; Korol, Aleksandr/A-6244-2014; Guo, Jun/O-5202-2015; Smirnova, Oxana/A-4401-2013; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Olshevskiy, Alexander/I-1580-2016; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Mora Herrera, Maria Clemencia/L-3893-2016; Grancagnolo, Sergio/J-3957-2015; spagnolo, stefania/A-6359-2012; Shmeleva, Alevtina/M-6199-2015; Camarri, Paolo/M-7979-2015; Gavrilenko, Igor/M-8260-2015; Tikhomirov, Vladimir/M-6194-2015; Chekulaev, Sergey/O-1145-2015; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; Carvalho, Joao/M-4060-2013; Mashinistov, Ruslan/M-8356-2015; Gonzalez de la Hoz, Santiago/E-2494-2016; Livan, Michele/D-7531-2012; Mitsou, Vasiliki/D-1967-2009; Joergensen, Morten/E-6847-2015; Riu, Imma/L-7385-2014; Cabrera Urban, Susana/H-1376-2015; Mir, Lluisa-Maria/G-7212-2015; Garcia, Jose /H-6339-2015; Della Pietra, Massimo/J-5008-2012; Cavalli-Sforza, Matteo/H-7102-2015; Ferrer, Antonio/H-2942-2015; Prokoshin, Fedor/E-2795-2012; Hansen, John/B-9058-2015; De, Kaushik/N-1953-2013; Sukharev, Andrey/A-6470-2014; O'Shea, Val/G-1279-2010; Lee, Jason/B-9701-2014; Robson, Aidan/G-1087-2011; Negrini, Matteo/C-8906-2014; Fabbri, Laura/H-3442-2012; Villa, Mauro/C-9883-2009; Kepka, Oldrich/G-6375-2014; Nemecek, Stanislav/G-5931-2014; Jakoubek, Tomas/G-8644-2014; Lokajicek, Milos/G-7800-2014; Staroba, Pavel/G-8850-2014; Kupco, Alexander/G-9713-2014; Andreazza, Attilio/E-5642-2011; Boyko, Igor/J-3659-2013; Kuleshov, Sergey/D-9940-2013; Anjos, Nuno/I-3918-2013; Kartvelishvili, Vakhtang/K-2312-2013; Dawson, Ian/K-6090-2013; Solfaroli Camillocci, Elena/J-1596-2012; Tudorache, Alexandra/L-3557-2013; Tudorache, Valentina/D-2743-2012; Marti-Garcia, Salvador/F-3085-2011; Wolters, Helmut/M-4154-2013; Warburton, Andreas/N-8028-2013; Stoicea, Gabriel/B-6717-2011; Brooks, William/C-8636-2013; Doyle, Anthony/C-5889-2009; Pina, Joao /C-4391-2012; Amorim, Antonio/C-8460-2013; Vanyashin, Aleksandr/H-7796-2013; Ferrando, James/A-9192-2012; Casadei, Diego/I-1785-2013; La Rosa, Alessandro/I-1856-2013; Moraes, Arthur/F-6478-2010; Smirnov, Sergei/F-1014-2011; Conde Muino, Patricia/F-7696-2011; Mikestikova, Marcela/H-1996-2014; Kuday, Sinan/C-8528-2014; Snesarev, Andrey/H-5090-2013; Svatos, Michal/G-8437-2014; Chudoba, Jiri/G-7737-2014; Veneziano, Stefano/J-1610-2012; Peleganchuk, Sergey/J-6722-2014; Santamarina Rios, Cibran/K-4686-2014; Bosman, Martine/J-9917-2014; Lei, Xiaowen/O-4348-2014; Demirkoz, Bilge/C-8179-2014; Ventura, Andrea/A-9544-2015 OI Petrucci, Fabrizio/0000-0002-5278-2206; Annovi, Alberto/0000-0002-4649-4398; Wemans, Andre/0000-0002-9669-9500; Cascella, Michele/0000-0003-2091-2501; Moorhead, Gareth/0000-0002-9299-9549; Gomes, Agostinho/0000-0002-5940-9893; Fassi, Farida/0000-0002-6423-7213; la rotonda, laura/0000-0002-6780-5829; Osculati, Bianca Maria/0000-0002-7246-060X; Amorim, Antonio/0000-0003-0638-2321; Santos, Helena/0000-0003-1710-9291; Coccaro, Andrea/0000-0003-2368-4559; Fiolhais, Miguel/0000-0001-9035-0335; Karyukhin, Andrey/0000-0001-9087-4315; Anjos, Nuno/0000-0002-0018-0633; Smestad, Lillian/0000-0002-0244-8736; Giordani, Mario/0000-0002-0792-6039; Abdelalim, Ahmed Ali/0000-0002-2056-7894; Capua, Marcella/0000-0002-2443-6525; Di Micco, Biagio/0000-0002-4067-1592; Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; Doria, Alessandra/0000-0002-5381-2649; Veloso, Filipe/0000-0002-5956-4244; Maneira, Jose/0000-0002-3222-2738; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Goncalo, Ricardo/0000-0002-3826-3442; Gauzzi, Paolo/0000-0003-4841-5822; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Monzani, Simone/0000-0002-0479-2207; Grancagnolo, Francesco/0000-0002-9367-3380; Korol, Aleksandr/0000-0001-8448-218X; Maio, Amelia/0000-0001-9099-0009; Guo, Jun/0000-0001-8125-9433; Smirnova, Oxana/0000-0003-2517-531X; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Olshevskiy, Alexander/0000-0002-8902-1793; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Grancagnolo, Sergio/0000-0001-8490-8304; spagnolo, stefania/0000-0001-7482-6348; Camarri, Paolo/0000-0002-5732-5645; Tikhomirov, Vladimir/0000-0002-9634-0581; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; Carvalho, Joao/0000-0002-3015-7821; Mashinistov, Ruslan/0000-0001-7925-4676; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Livan, Michele/0000-0002-5877-0062; Mitsou, Vasiliki/0000-0002-1533-8886; Joergensen, Morten/0000-0002-6790-9361; Riu, Imma/0000-0002-3742-4582; Mir, Lluisa-Maria/0000-0002-4276-715X; Della Pietra, Massimo/0000-0003-4446-3368; Ferrer, Antonio/0000-0003-0532-711X; Prokoshin, Fedor/0000-0001-6389-5399; Hansen, John/0000-0002-8422-5543; De, Kaushik/0000-0002-5647-4489; O'Shea, Val/0000-0001-7183-1205; Lee, Jason/0000-0002-2153-1519; Negrini, Matteo/0000-0003-0101-6963; Fabbri, Laura/0000-0002-4002-8353; Villa, Mauro/0000-0002-9181-8048; Andreazza, Attilio/0000-0001-5161-5759; Boyko, Igor/0000-0002-3355-4662; Kuleshov, Sergey/0000-0002-3065-326X; Solfaroli Camillocci, Elena/0000-0002-5347-7764; Wolters, Helmut/0000-0002-9588-1773; Warburton, Andreas/0000-0002-2298-7315; Stoicea, Gabriel/0000-0002-7511-4614; Brooks, William/0000-0001-6161-3570; Doyle, Anthony/0000-0001-6322-6195; Pina, Joao /0000-0001-8959-5044; Vanyashin, Aleksandr/0000-0002-0367-5666; Ferrando, James/0000-0002-1007-7816; La Rosa, Alessandro/0000-0001-6291-2142; Moraes, Arthur/0000-0002-5157-5686; Smirnov, Sergei/0000-0002-6778-073X; Conde Muino, Patricia/0000-0002-9187-7478; Mikestikova, Marcela/0000-0003-1277-2596; Kuday, Sinan/0000-0002-0116-5494; Svatos, Michal/0000-0002-7199-3383; Veneziano, Stefano/0000-0002-2598-2659; Peleganchuk, Sergey/0000-0003-0907-7592; Santamarina Rios, Cibran/0000-0002-9810-1816; Bosman, Martine/0000-0002-7290-643X; Lei, Xiaowen/0000-0002-2564-8351; Ventura, Andrea/0000-0002-3368-3413 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET; ERC; European Union; IN2P3-CNRS; CFA-OSM/IRFU; Frame; GNAS, Georgia; BMBF, Germany; DFG, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; ISF, Israel; MINERVA, Israel; CIF, Israel; DIP, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; GRICES, Portugal; FCT, Portugal; MERYS (MECTS), Romania; MES of Russia; ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MVZT, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SFR; SNSF; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America; Canton of Bern, Switzerland; Canton of Geneva, Switzerland FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF, Austria: ANAS, Azerbaijan; SSTC, Belarus: CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China: COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET and ERC, European Union; IN2P3-CNRS, CFA-OSM/IRFU, Frame; GNAS, Georgia; BMBF, DFG, MPG and AvH Foundation, Germany; GSRT, Greece; ISF, MINERVA, CIF, DIP and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW, Poland; GRICES and FCT, Portugal;,MERYS (MECTS), Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MVZT, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC and Wallenberg Foundation, Sweden; SFR, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. NR 81 TC 11 Z9 11 U1 4 U2 102 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD NOV PY 2012 IS 11 AR 138 DI 10.1007/JHEP11(2012)138 PG 46 WC Physics, Particles & Fields SC Physics GA 056JL UT WOS:000312484500008 ER PT J AU Buras, AJ Gorbahn, M Haisch, U Neirste, U AF Buras, Andrzej J. Gorbahn, Martin Haisch, Ulrich Neirste, Ulrich TI charm quark contribution to K+ -> pi(+)nu(nu)over-bar at next-to-next-to-leading order (vol 11, 002, 2006) SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Correction AB We correct the treatment of anomalous triangle diagrams occuring in the effective theory in which the heavy top quark is integrated out. To this end we determine the initial conditions and anomalous dimensions of the operator describing the Z-mediated coupling of neutrinos to quarks and further rectify the bilocal renormalization group evolution. Our changes affect the charm-quark contribution P-c(X) at the next-to-leading and next-to-next-to-leading orders, but are numerically negligible as they amout to relative shifts below a permille. C1 [Buras, Andrzej J.] Tech Univ Munich, Dept Phys, D-85748 Garching, Germany. [Gorbahn, Martin] Univ Durham, IPPP, Dept Phys, Durham DH1 3LE, England. [Gorbahn, Martin; Neirste, Ulrich] Univ Karlsruhe, Inst Theoret Teilchenphys, D-76128 Karlsruhe, Germany. [Haisch, Ulrich; Neirste, Ulrich] Fermilab Natl Accelerator Lab, Dept Theoret Phys, Batavia, IL 60510 USA. [Haisch, Ulrich] Univ Zurich, Inst Theoret Phys, CH-8057 Zurich, Switzerland. RP Buras, AJ (reprint author), Tech Univ Munich, Dept Phys, D-85748 Garching, Germany. EM andrzej.buras@tum.de; mgorbahn@particle.uni-karlsruhe.de; uhaisch@physik.unizh.ch; nierste@particle.uni-karlsruhe.de NR 3 TC 4 Z9 4 U1 0 U2 1 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD NOV PY 2012 IS 11 AR 167 DI 10.1007/JHEP11(2012)167 PG 5 WC Physics, Particles & Fields SC Physics GA 056JL UT WOS:000312484500036 ER PT J AU Campbell, JM Hartanto, HB Williams, C AF Campbell, John M. Hartanto, Heribertus B. Williams, Ciaran TI Next-to-leading order predictions for Z gamma plus jet and Z gamma gamma final states at the LHC SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE NLO Computations; Hadronic Colliders ID ONE-LOOP AMPLITUDES; HADRON COLLIDERS; W-GAMMA; ELECTROWEAK CORRECTIONS; CROSS-SECTIONS; QCD; COUPLINGS; PHOTONS; TEV AB We present next-to-leading order predictions for final states containing leptons produced through the decay of a Z boson in association with either a photon and a jet, or a, pair of photons. The effect of photon radiation from the final state leptons is included and we also allow for contributions arising from fragmentation processes. Phenomenological studies are presented for the LHC in the case of final states containing charged leptons and in the case of neutrinos. We also use the procedure introduced by Stewart and Tackmann to provide a reliable estimate of the scale uncertainty inherent in our theoretical calculations of jet-binned Z gamma cross sections. These computations have been implemented in the public code MCFM. C1 [Campbell, John M.; Hartanto, Heribertus B.; Williams, Ciaran] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Hartanto, Heribertus B.] Florida State Univ, Dept Phys, Tallahassee, FL 32306 USA. RP Campbell, JM (reprint author), Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. EM johnmc@fnal.gov; hhartanto@hep.fsu.edu; ciaran@fnal.gov FU U.S. Department of Energy [DE-FG02-97ER41022]; Fermilab Fellowship in Theoretical Physics; United States Department of Energy [DE-AC02-07CH11359] FX We thank Keith Ellis and Al Goshaw for useful discussions. HBH is supported by the U.S. Department of Energy under grant DE-FG02-97ER41022 and the Fermilab Fellowship in Theoretical Physics. Fermilab is operated by Fermi Research Alliance, LLC under Contract No. DE-AC02-07CH11359 with the United States Department of Energy. NR 38 TC 9 Z9 9 U1 2 U2 4 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. 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CA CMS Collaboration TI Search for new physics with long-lived particles decaying to photons and missing energy in pp collisions at root s=7 TeV SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering ID MEDIATED SUPERSYMMETRY BREAKING; COLLIDERS AB A search is performed for long-lived neutral particles decaying into a photon and invisible particles. An example of such a signature is the decay of the lightest neutralino with nonzero lifetime into a gravitino and a photon in gauge-mediated supersymmetry, with the neutralino as the next-to-lightest supersymmetric particle and the gravitino as the lightest. The search uses events containing photons, missing transverse energy, and jets. The impact parameter of the photon relative to the beam-beam collision point can be reconstructed using converted photons. The method is sensitive to lifetimes of the order of 0.1 to ins. The data sample corresponds to an integrated luminosity of 2.23 fb(-1) in pp collisions at root s = 7 TeV, recorded in the first part of 2011 by the CMS experiment at the LHC. Cross-section limits are presented on pair production for such particles, each of which decays into a photon and invisible particles. The observed 95% confidence level limits vary between 0.11 and 0.21 pb, depending on the neutral particle lifetime. C1 [Chatrchyan, S.; Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Aguilo, E.; Bergauer, T.; Dragicevic, M.; Eroe, J.; Fabjan, C.; Friedl, M.; Fruehwirth, R.; Ghete, V. M.; Hammer, J.; Hoermann, N.; Hrubec, J.; Jeitler, M.; Kiesenhofer, W.; Knuenz, V.; Krammer, M.; Kraetschmer, I.; Liko, D.; Mikulec, I.; Pernicka, M.; Rahbaran, B.; Rohringer, C.; Rohringer, H.; Schoefbeck, R.; Strauss, J.; Taurok, A.; Waltenberger, W.; Walzel, G.; Widl, E.; Wulz, C. -E.] OeAW, Inst Hochenergiephys, Vienna, Austria. 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B.; Parida, B.; Sudhakar, K.; Wickramage, N.] Tata Inst Fundamental Res, EHEP, Mumbai 400005, Maharashtra, India. [Banerjee, S.; Guchait, M.; Dugad, S.] Tata Inst Fundamental Res, HECR, Mumbai 400005, Maharashtra, India. [Arfaei, H.; Bakhshiansohi, H.; Etesami, S. M.; Fahim, A.; Hashemi, M.; Hesari, H.; Jafari, A.; Khakzad, M.; Najafabadi, M. Mohammadi; Mehdiabadi, S. Paktinat; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; Colaleo, A.; Creanza, D.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Lusito, L.; Maggi, G.; Maggi, M.; Marangelli, B.; My, S.; Nuzzo, S.; Pacifico, N.; Pompili, A.; Pugliese, G.; Selvaggi, G.; Silvestris, L.; Singh, G.; Zito, G.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; De Palma, M.; Lusito, L.; Marangelli, B.; Nuzzo, S.; Pacifico, N.; Pompili, A.; Selvaggi, G.; Singh, G.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Meneghelli, M.; Montanari, A.; Navarria, F. L.; Odorici, F.; Perrotta, A.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G.; Travaglini, R.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Capiluppi, P.; Castro, A.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Meneghelli, M.; Navarria, F. L.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gallo, E.; Gonzi, S.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gonzi, S.] Univ Florence, Florence, Italy. [Fabbri, F.; Benussi, L.; Bianco, S.; Colafranceschi, S.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Fabbricatore, P.; Musenich, R.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Benaglia, A.; De Guio, F.; Di Matteo, L.; Fiorendi, S.; Gennai, S.; Ghezzi, A.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Massironi, A.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; Sala, S.; de Fatis, T. Tabarelli] Ist Nazl Fis Nucl, Sez Milano Bicocca, I-20133 Milan, Italy. [Benaglia, A.; De Guio, F.; Di Matteo, L.; Fiorendi, S.; Ghezzi, A.; Manzoni, R. A.; Martelli, A.; Massironi, A.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Montoya, C. A. Carrillo; Cavallo, N.; De Cosa, A.; Dogangun, O.; Fabozzi, F.; Iorio, A. O. M.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [De Cosa, A.; Dogangun, O.; Merola, M.] Univ Naples Federico II, Naples, Italy. [Azzi, P.; Bacchetta, N.; Bellan, P.; Bisello, D.; Branca, A.; Checchia, P.; Dorigo, T.; Dosselli, U.; Gasparini, F.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Lazzizzera, I.; Margoni, M.; Meneguzzo, A. T.; Nespolo, M.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Vanini, S.; Zotto, P.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Bellan, P.; Bisello, D.; Gasparini, F.; Margoni, M.; Meneguzzo, A. T.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Vanini, S.; Zotto, P.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.; Lazzizzera, I.] Univ Trento Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Torre, P.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Torre, P.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Biasini, M.; Bilei, G. M.; Fano, L.; Lariccia, P.; Lucaroni, A.; Mantovani, G.; Menichelli, M.; Nappi, A.; Romeo, F.; Saha, A.; Santocchia, A.; Spiezia, A.; Taroni, S.; Pioppi, M.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Biasini, M.; Fano, L.; Lariccia, P.; Lucaroni, A.; Mantovani, G.; Nappi, A.; Romeo, F.; Santocchia, A.; Spiezia, A.; Taroni, S.; Pioppi, M.] Univ Perugia, I-06100 Perugia, Italy. [Azzurri, P.; Bagliesi, G.; Boccali, T.; Broccolo, G.; Castaldi, R.; D'Agnolo, R. T.; Dell'Orso, R.; Fiori, F.; Foa, L.; Giassi, A.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Fiori, F.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Azzurri, P.; Broccolo, G.; D'Agnolo, R. T.; Foa, L.; Ligabue, F.; Rolandi, G.] Ist Nazl Fis Nucl, Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Del Re, D.; Diemoz, M.; Grassi, M.; Longo, E.; Meridiani, P.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Paramatti, R.; Rahatlou, S.; Sigamani, M.; Soffi, L.; Rovelli, C.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; Del Re, D.; Grassi, M.; Longo, E.; Micheli, F.; Nourbakhsh, S.; Organtini, G.; Rahatlou, S.; Soffi, L.; Rovelli, C.] Univ Roma La Sapienza, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Biino, C.; Cartiglia, N.; De Remigis, P.; Demaria, N.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Pastrone, N.; Pelliccioni, M.; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Pereira, A. Vilela; Acosta, D.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Costa, M.; Migliore, E.; Monaco, V.; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; Marone, M.; Montanino, D.; Penzo, A.; Schizzi, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; Marone, M.; Montanino, D.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Heo, S. G.; Kim, T. Y.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Chang, S.; Kim, D. H.; Kim, G. N.; Kong, D. J.; Park, H.; Ro, S. R.; Son, D. C.; Son, T.; Kamon, T.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, J. Y.; Kim, Zero J.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, T. J.; Lee, K. S.; Moon, D. H.; Park, S. K.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Cho, Y.; Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. S.; Kwon, E.; Lee, B.; Lee, J.; Lee, S.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Bilinskas, M. J.; Grigelionis, I.; Janulis, M.; Juodagalvis, A.] Vilnius State Univ, Vilnius, Lithuania. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Lopez-Fernandez, R.; Magana Villalba, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.; Reyes-Santos, M. A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Bell, A. J.; Butler, P. H.; Doesburg, R.; Reucroft, S.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Ansari, M. H.; Asghar, M. I.; Hoorani, H. R.; Khalid, S.; Khan, W. 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[Evstyukhin, S.; Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Matveev, V.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow, Russia. [Epshteyn, V.; Erofeeva, M.; Gavrilov, V.; Kossov, M.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Stolin, V.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Zhukov, V.; Katkov, I.; Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Markina, A.; Obraztsov, S.; Perfilov, M.; Petrushanko, S.; Popov, A.; Sarycheva, L.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Grishin, V.; Kachanov, V.; Konstantinov, D.; Korablev, A.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade, Serbia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Alcaraz Maestre, J.; Arce, P.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.; Willmott, C.] CIEMAT, Madrid, Spain. [Albajar, C.; Codispoti, G.; de Troconiz, J. F.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.; Piedra Gomez, J.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Chuang, S. H.; Duarte Campderros, J.; Felcini, M.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Graziano, A.; Jorda, C.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Sobron Sanudo, M.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Genchev, V.; Iaydjiev, P.; Puljak, I.; Chierici, R.; Guthoff, M.; Hauth, T.; Sharma, A.; Mohanty, A. K.; Calabria, C.; De Filippis, N.; Fasanella, D.; Meneghelli, M.; Di Matteo, L.; Gennai, S.; Massironi, A.; De Cosa, A.; Paolucci, P.; Bacchetta, N.; Branca, A.; Nespolo, M.; Tosi, M.; Lucaroni, A.; Fiori, F.; Squillacioti, P.; Tonelli, G.; Grassi, M.; Meridiani, P.; Mariotti, C.; Musich, M.; Marone, M.; Montanino, D.; Grishin, V.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Perez, J. A. Coarasa; D'Enterria, D.; Dabrowski, A.; De Roeck, A.; Di Guida, S.; Dobson, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Frisch, B.; Funk, W.; Georgiou, G.; Giffels, M.; Gigi, D.; Gill, K.; Giordano, D.; Giunta, M.; Glege, F.; Garrido, R. Gomez-Reino; Govoni, P.; Gowdy, S.; Guida, R.; Hansen, M.; Harris, P.; Hartl, C.; Harvey, J.; Hegner, B.; Hinzmann, A.; Innocente, V.; Janot, P.; Kaadze, K.; Karavakis, E.; Kousouris, K.; Lecoq, P.; Lee, Y. -J.; Lenzi, P.; Lourenco, C.; Magini, N.; Maeki, T.; Malberti, M.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moser, R.; Mozer, M. U.; Mulders, M.; Musella, P.; Nesvold, E.; Orimoto, T.; Orsini, L.; Cortezon, E. Palencia; Perez, E.; Perrozzi, L.; Petrilli, A.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Piparo, D.; Polese, G.; Quertenmont, L.; Racz, A.; Reece, W.; Antunes, J. Rodrigues; Rolandi, G.; Rovelli, C.; Rovere, M.; Sakulin, H.; Santanastasio, F.; Schaefer, C.; Schwick, C.; Segoni, I.; Sekmen, S.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Tsirou, A.; Veres, G. I.; Vlimant, J. R.; Woehri, H. K.; Worm, S. D.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Gabathuler, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Meier, F.; Renker, D.; Rohe, T.; Sibille, J.; Naegeli, C.] Paul Scherrer Inst, Villigen, Switzerland. [Baeni, L.; Bortignon, P.; Buchmann, M. A.; Casal, B.; Chanon, N.; Deisher, A.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eugster, J.; Freudenreich, K.; Grab, C.; Hits, D.; Lecomte, P.; Lustermann, W.; Marini, A. C.; del Arbol, P. Martinez Ruiz; Mohr, N.; Moortgat, F.; Naegeli, C.; Nef, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pape, L.; Pauss, F.; Peruzzi, M.; Ronga, F. J.; Rossini, M.; Sala, L.; Sanchez, A. K.; Starodumov, A.; Stieger, B.; Takahashi, M.; Tauscher, L.; Thea, A.; Theofilatos, K.; Treille, D.; Urscheler, C.; Wallny, R.; Weber, H. A.; Wehrli, L.] ETH, Inst Particle Phys, Zurich, Switzerland. [Amsler, C.; Chiochia, V.; De Visscher, S.; Favaro, C.; Rikova, M. Ivova; Mejias, B. Millan; Otiougova, P.; Robmann, P.; Snoek, H.; Tupputi, S.; Verzetti, M.] Univ Zurich, Zurich, Switzerland. [Chang, Y. H.; Chen, K. H.; Kuo, C. M.; Li, S. W.; Lin, W.; Liu, Z. K.; Lu, Y. J.; Mekterovic, D.; Singh, A. P.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Dietz, C.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wan, X.; Wang, M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Karaman, T.; Karapinar, G.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, L. N.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Yildirim, E.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey. [Cankocak, K.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Bostock, F.; Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Kreczko, L.; Metson, S.; Newbold, D. M.; Nirunpong, K.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Worm, S. D.; Newbold, D. M.; Basso, L.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Jackson, J.; Kennedy, B. W.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Womersley, W. J.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Bainbridge, R.; Ball, G.; Beuselinck, R.; Buchmuller, O.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Papageorgiou, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Ryan, M. J.; Seez, C.; Sharp, P.; Sparrow, A.; Stoye, M.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.; Whyntie, T.] Univ London Imperial Coll Sci Technol & Med, London, England. [Chadwick, M.; Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Hatakeyama, K.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; St John, J.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Bhattacharya, S.; Alimena, J.; Cutts, D.; Ferapontov, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Nguyen, D.; Segala, M.; Sinthuprasith, T.; Speer, T.; Tsang, K. V.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Dolen, J.; Erbacher, R.; Gardner, M.; Houtz, R.; Ko, W.; Kopecky, A.; Lander, R.; Miceli, T.; Pellett, D.; Ricci-tam, F.; Rutherford, B.; Searle, M.; Smith, J.; Squires, M.; Tripathi, M.; Sierra, R. Vasquez] Univ Calif Davis, Davis, CA 95616 USA. [Weber, M.; Andreev, V.; Felcini, M.; Cline, D.; Cousins, R.; Duris, J.; Erhan, S.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Plager, C.; Rakness, G.; Schlein, P.; Traczyk, P.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Liu, H.; Babb, J.; Clare, R.; Dinardo, M. E.; Ellison, J.; Gary, J. W.; Giordano, F.; Hanson, G.; Jeng, G. Y.; Long, O. R.; Luthra, A.; Nguyen, H.; Paramesvaran, S.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sharma, V.; Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; Evans, D.; Golf, F.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Macneill, I.; Mangano, B.; Padhi, S.; Palmer, C.; Petrucciani, G.; Pieri, M.; Sani, M.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bellan, R.; Campagnari, C.; D'Alfonso, M.; Danielson, T.; Flowers, K.; Geffert, P.; Incandela, J.; Justus, C.; Kalavase, P.; Koay, S. A.; Kovalskyi, D.; Krutelyov, V.; Lowette, S.; Mccoll, N.; Pavlunin, V.; Rebassoo, F.; Ribnik, J.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dias, F. A.; Dubinin, M.; Apresyan, A.; Bornheim, A.; Chen, Y.; Di Marco, E.; Duarte, J.; Gataullin, M.; Ma, Y.; Mott, A.; Newman, H. B.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Veverka, J.; Wilkinson, R.; Xie, S.; Yang, Y.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Akgun, B.; Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Liu, Y. F.; Paulini, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Edelmaier, C. J.; Ford, W. T.; Gaz, A.; Heyburn, B.; Lopez, E. Luiggi; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Eggert, N.; Gibbons, L. K.; Heltsley, B.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Vaughan, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bloch, I.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Green, D.; Gutsche, O.; Hanlon, J.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Kilminster, B.; Klima, B.; Kunori, S.; Kwan, S.; Leonidopoulos, C.; Linacre, J.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Tan, P.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Wu, W.; Yang, F.; Yumiceva, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Piedra Gomez, J.; Acosta, D.; Avery, P.; Bourilkov, D.; Chen, M.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Drozdetskiy, A.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Gartner, J.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Remington, R.; Rinkevicius, A.; Sellers, P.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Hewamanage, S.; Lebolo, L. M.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Gleyzer, S. V.; Haas, J.; Hagopian, S.; Hagopian, V.; Jenkins, M.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Vodopiyanov, I.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Anghel, I. M.; Apanasevich, L.; Bai, Y.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Callner, J.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Lacroix, F.; Malek, M.; O'Brien, C.; Silkworth, C.; Strom, D.; Varelas, N.] Univ Illinois, Chicago, IL USA. [Ozturk, S.; Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Duru, F.; Griffiths, S.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Newsom, C. R.; Norbeck, E.; Onel, Y.; Ozok, F.; Sen, S.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Giurgiu, G.; Gritsan, A. V.; Guo, Z. J.; Hu, G.; Maksimovic, P.; Rappoccio, S.; Swartz, M.; Whitbeck, A.] Johns Hopkins Univ, Baltimore, MD USA. [Sibille, J.; Baringer, P.; Bean, A.; Benelli, G.; Grachov, O.; Iii, R. P. Kenny; Murray, M.; Noonan, D.; Sanders, S.; Stringer, R.; Tinti, G.; Wood, J. S.; Zhukova, V.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Bolton, T.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Boutemeur, M.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kirn, M.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Peterman, A.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.; Twedt, E.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Bauer, G.; Bendavid, J.; Busza, W.; Butz, E.; Cali, I. A.; Chan, M.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Hahn, K. A.; Kim, Y.; Klute, M.; Krajczar, K.; Luckey, P. D.; Ma, T.; Nahn, S.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Rudolph, M.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Sung, K.; Velicanu, D.; Wenger, E. A.; Wolf, R.; Wyslouch, B.; Yang, M.; Yilmaz, Y.; Yoon, A. S.; Zanetti, M.] MIT, Cambridge, MA 02139 USA. [Cooper, S. I.; Dahmes, B.; De Benedetti, A.; Franzoni, G.; Gude, A.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Sasseville, M.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Cremaldi, L. M.; Kroeger, R.; Perera, L.; Rahmat, R.; Sanders, D. A.] Univ Mississippi, University, MS 38677 USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Butt, J.; Claes, D. R.; Dominguez, A.; Eads, M.; Keller, J.; Kravchenko, I.; Lazo-Flores, J.; Malbouisson, H.; Malik, S.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Baur, U.; Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Kumar, A.; Shipkowski, S. P.; Smith, K.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Nash, D.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Anastassov, A.; Kubik, A.; Mucia, N.; Odell, N.; Ofierzynski, R. A.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Antonelli, L.; Berry, D.; Brinkerhoff, A.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kolb, J.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Morse, D. M.; Pearson, T.; Planer, M.; Ruchti, R.; Slaunwhite, J.; Valls, N.; Wayne, M.; Wolf, M.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Bylsma, B.; Durkin, L. S.; Hill, C.; Kotov, K.; Ling, T. Y.; Puigh, D.; Rodenburg, M.; Vuosalo, C.; Williams, G.; Winer, B. L.] Ohio State Univ, Columbus, OH 43210 USA. [Adam, N.; Berry, E.; Elmer, P.; Gerbaudo, D.; Halyo, V.; Hebda, P.; Hegeman, J.; Hunt, A.; Jindal, P.; Pegna, D. Lopes; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Raval, A.; Safdi, B.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Acosta, J. G.; Brownson, E.; Huang, X. T.; Lopez, A.; Mendez, H.; Oliveros, S.; Vargas, J. E. Ramirez; Zatserklyaniy, A.] Univ Puerto Rico, Mayaguez, PR USA. [Alagoz, E.; Barnes, V. E.; Benedetti, D.; Bolla, G.; Bortoletto, D.; De Mattia, M.; Everett, A.; Hu, Z.; Jones, M.; Koybasi, O.; Kress, M.; Laasanen, A. T.; Leonardo, N.; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Marono, M. Vidal; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Guragain, S.; Parashar, N.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Boulahouache, C.; Ecklund, K. M.; Geurts, F. J. M.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; Chung, Y. S.; Covarelli, R.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Miner, D. C.; Vishnevskiy, D.; Zielinski, M.] Univ Rochester, Rochester, NY 14627 USA. [Malik, S.; Bhatti, A.; Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Lath, A.; Panwalkar, S.; Park, M.; Patel, R.; Rekovic, V.; Robles, J.; Rose, K.; Salur, S.; Schnetzer, S.; Seitz, C.; Somalwar, S.; Stone, R.; Thomas, S.] Rutgers State Univ, Piscataway, NJ USA. [Cerizza, G.; Hollingsworth, M.; Spanier, S.; Yang, Z. C.; York, A.] Univ Tennessee, Knoxville, TN USA. [Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Khotilovich, V.; Montalvo, R.; Osipenkov, I.; Pakhotin, Y.; Perloff, A.; Roe, J.; Safonov, A.; Sakuma, T.; Sengupta, S.; Suarez, I.; Tatarinov, A.; Toback, D.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Jeong, C.; Kovitanggoon, K.; Lee, S. W.; Libeiro, T.; Roh, Y.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Appelt, E.; Delannoy, A. G.; Florez, C.; Greene, S.; Gurrola, A.; Johns, W.; Johnston, C.; Kurt, P.; Maguire, C.; Melo, A.; Sharma, M.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.] Vanderbilt Univ, Nashville, TN USA. [Arenton, M. W.; Balazs, M.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Lin, C.; Neu, C.; Wood, J.; Yohay, R.] Univ Virginia, Charlottesville, VA USA. [Gollapinni, S.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sakharov, A.] Wayne State Univ, Detroit, MI USA. [Anderson, M.; Belknap, D.; Borrello, L.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Gray, L.; Grogg, K. S.; Grothe, M.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Klukas, J.; Lanaro, A.; Lazaridis, C.; Leonard, J.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Palmonari, F.; Pierro, G. A.; Ross, I.; Savin, A.; Smith, W. H.; Swanson, J.] Univ Wisconsin, Madison, WI 53706 USA. [Fabjan, C.; Fruehwirth, R.; Jeitler, M.; Krammer, M.; Wulz, C. -E.] Vienna Univ Technol, A-1040 Vienna, Austria. [Anjos, T. S.; Bernardes, C. A.; Gregores, E. M.; Mercadante, P. G.] Univ Fed ABC, Santo Andre, Brazil. [Assran, Y.] Suez Canal Univ, Suez, Egypt. [Elgammal, S.; Khalil, S.] Zewail City Sci & Technol, Zewail, Egypt. [Kamel, A. Ellithi] Cairo Univ, Cairo, Egypt. [Mahmoud, M. A.] Fayoum Univ, Al Fayyum, Egypt. [Radi, A.] British Univ, Cairo, Egypt. [Agram, J. -L.; Conte, E.; Drouhin, F.; Fontaine, J. -C.] Univ Haute Alsace, Mulhouse, France. [Bergholz, M.; Lohmann, W.; Schmidt, R.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Vesztergombi, G.; Veres, G. I.] Eotvos Lorand Univ, Budapest, Hungary. [Maity, M.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Bakhshiansohi, H.; Fahim, A.; Jafari, A.] Sharif Univ Technol, Tehran, Iran. [Etesami, S. M.; Zeinali, M.] Isfahan Univ Technol, Esfahan, Iran. [Safarzadeh, B.] Islamic Azad Univ, Sci & Res Branch, Plasma Phys Res Ctr, Tehran, Iran. [Colafranceschi, S.] Univ Roma, Fac Ingn, Rome, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata, I-85100 Potenza, Italy. [Meola, S.] Univ Guglielmo Marconi, Rome, Italy. [Martini, L.] Univ Siena, I-53100 Siena, Italy. [Serban, A. T.] Univ Bucharest, Fac Phys, Bucharest, Romania. [Bakirci, M. N.; Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey. [Cerci, S.; Cerci, D. Sunar; Tali, B.] Adiyaman Univ, Adiyaman, Turkey. 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RI Sguazzoni, Giacomo/J-4620-2015; Ligabue, Franco/F-3432-2014; Fassi, Farida/F-3571-2016; Hernandez Calama, Jose Maria/H-9127-2015; Menasce, Dario Livio/A-2168-2016; Bargassa, Pedrame/O-2417-2016; Kirakosyan, Martin/N-2701-2015; Gulmez, Erhan/P-9518-2015; Seixas, Joao/F-5441-2013; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Gerbaudo, Davide/J-4536-2012; My, Salvatore/I-5160-2015; Matorras, Francisco/I-4983-2015; Ragazzi, Stefano/D-2463-2009; Dremin, Igor/K-8053-2015; Hoorani, Hafeez/D-1791-2013; Leonidov, Andrey/M-4440-2013; Andreev, Vladimir/M-8665-2015; TUVE', Cristina/P-3933-2015; KIM, Tae Jeong/P-7848-2015; Arce, Pedro/L-1268-2014; Flix, Josep/G-5414-2012; Azarkin, Maxim/N-2578-2015; Paganoni, Marco/A-4235-2016; Benussi, Luigi/O-9684-2014; Dahms, Torsten/A-8453-2015; Grandi, Claudio/B-5654-2015; Leonidov, Andrey/P-3197-2014; Bernardes, Cesar Augusto/D-2408-2015; Lazzizzera, Ignazio/E-9678-2015; Sen, Sercan/C-6473-2014; D'Alessandro, Raffaello/F-5897-2015; Belyaev, Alexander/F-6637-2015; Stahl, Achim/E-8846-2011; Trocsanyi, Zoltan/A-5598-2009; Konecki, Marcin/G-4164-2015; Bedoya, Cristina/K-8066-2014; Gribushin, Andrei/J-4225-2012; Cerrada, Marcos/J-6934-2014; Azzi, Patrizia/H-5404-2012; Calderon, Alicia/K-3658-2014; de la Cruz, Begona/K-7552-2014; Scodellaro, Luca/K-9091-2014; Josa, Isabel/K-5184-2014; Calvo Alamillo, Enrique/L-1203-2014; Paulini, Manfred/N-7794-2014; Vogel, Helmut/N-8882-2014; Marinho, Franciole/N-8101-2014; Ferguson, Thomas/O-3444-2014; Venturi, Andrea/J-1877-2012; Wimpenny, Stephen/K-8848-2013; Markina, Anastasia/E-3390-2012; Dogangun, Oktay/L-9252-2013; Marlow, Daniel/C-9132-2014; de Jesus Damiao, Dilson/G-6218-2012; Oguri, Vitor/B-5403-2013; Janssen, Xavier/E-1915-2013; Bartalini, Paolo/E-2512-2014; Santoro, Alberto/E-7932-2014; Codispoti, Giuseppe/F-6574-2014; Max, Mad/E-5238-2010; Novaes, Sergio/D-3532-2012; Wulz, Claudia-Elisabeth/H-5657-2011; Fruhwirth, Rudolf/H-2529-2012; Rolandi, Luigi (Gigi)/E-8563-2013; Montanari, Alessandro/J-2420-2012; Raidal, Martti/F-4436-2012; Tomei, Thiago/E-7091-2012; Zalewski, Piotr/H-7335-2013; Tinti, Gemma/I-5886-2013; Ivanov, Andrew/A-7982-2013; Hill, Christopher/B-5371-2012; Liu, Sheng/K-2815-2013; Zhukov, Valery/K-3615-2013; Mundim, Luiz/A-1291-2012; De La Cruz Burelo, Eduard/B-9802-2013; Petrushanko, Sergey/D-6880-2012; Santaolalla, Javier/C-3094-2013; Alves, Gilvan/C-4007-2013; Tinoco Mendes, Andre David/D-4314-2011; Dudko, Lev/D-7127-2012; Mercadante, Pedro/K-1918-2012; Lokhtin, Igor/D-7004-2012; tosi, mia/J-5777-2012; Della Ricca, Giuseppe/B-6826-2013; Kadastik, Mario/B-7559-2008 OI Ciulli, Vitaliano/0000-0003-1947-3396; Fiorendi, Sara/0000-0003-3273-9419; Martelli, Arabella/0000-0003-3530-2255; Gonzi, Sandro/0000-0003-4754-645X; Levchenko, Petr/0000-0003-4913-0538; Heath, Helen/0000-0001-6576-9740; Safdi, Benjamin R./0000-0001-9531-1319; Sguazzoni, Giacomo/0000-0002-0791-3350; Ligabue, Franco/0000-0002-1549-7107; Diemoz, Marcella/0000-0002-3810-8530; Tricomi, Alessia Rita/0000-0002-5071-5501; Fassi, Farida/0000-0002-6423-7213; Heredia De La Cruz, Ivan/0000-0002-8133-6467; Ghezzi, Alessio/0000-0002-8184-7953; bianco, stefano/0000-0002-8300-4124; Demaria, Natale/0000-0003-0743-9465; Benaglia, Andrea Davide/0000-0003-1124-8450; Covarelli, Roberto/0000-0003-1216-5235; Vieira de Castro Ferreira da Silva, Pedro Manuel/0000-0002-5725-041X; Hernandez Calama, Jose Maria/0000-0001-6436-7547; Bean, Alice/0000-0001-5967-8674; Longo, Egidio/0000-0001-6238-6787; Di Matteo, Leonardo/0000-0001-6698-1735; Baarmand, Marc/0000-0002-9792-8619; Boccali, Tommaso/0000-0002-9930-9299; Menasce, Dario Livio/0000-0002-9918-1686; Bargassa, Pedrame/0000-0001-8612-3332; Attia Mahmoud, Mohammed/0000-0001-8692-5458; Bilki, Burak/0000-0001-9515-3306; Gulmez, Erhan/0000-0002-6353-518X; Seixas, Joao/0000-0002-7531-0842; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Gerbaudo, Davide/0000-0002-4463-0878; My, Salvatore/0000-0002-9938-2680; Matorras, Francisco/0000-0003-4295-5668; Ragazzi, Stefano/0000-0001-8219-2074; TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; Arce, Pedro/0000-0003-3009-0484; Flix, Josep/0000-0003-2688-8047; Paganoni, Marco/0000-0003-2461-275X; Benussi, Luigi/0000-0002-2363-8889; Dahms, Torsten/0000-0003-4274-5476; Grandi, Claudio/0000-0001-5998-3070; Lazzizzera, Ignazio/0000-0001-5092-7531; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Belyaev, Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279; Konecki, Marcin/0000-0001-9482-4841; Bedoya, Cristina/0000-0001-8057-9152; Cerrada, Marcos/0000-0003-0112-1691; Azzi, Patrizia/0000-0002-3129-828X; Scodellaro, Luca/0000-0002-4974-8330; Calvo Alamillo, Enrique/0000-0002-1100-2963; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Marinho, Franciole/0000-0002-7327-0349; Ferguson, Thomas/0000-0001-5822-3731; Wimpenny, Stephen/0000-0003-0505-4908; Dogangun, Oktay/0000-0002-1255-2211; de Jesus Damiao, Dilson/0000-0002-3769-1680; Codispoti, Giuseppe/0000-0003-0217-7021; Max, Mad/0000-0001-6966-6829; Novaes, Sergio/0000-0003-0471-8549; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Rolandi, Luigi (Gigi)/0000-0002-0635-274X; Montanari, Alessandro/0000-0003-2748-6373; Tomei, Thiago/0000-0002-1809-5226; Ivanov, Andrew/0000-0002-9270-5643; Hill, Christopher/0000-0003-0059-0779; Mundim, Luiz/0000-0001-9964-7805; De La Cruz Burelo, Eduard/0000-0002-7469-6974; Tinoco Mendes, Andre David/0000-0001-5854-7699; Dudko, Lev/0000-0002-4462-3192; Della Ricca, Giuseppe/0000-0003-2831-6982; FU FMSR (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MES (Bulgaria); CERN; CAS (China); MoST (China); NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); MoER [SF0690030s09]; ERDF (Estonia); Academy of Finland Finland; MEC Finland; HIP (Finland); CEA (France); CNRS/IN2P3 (France); BMBF (Germany); DFG (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NKTH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF (Korea); WCU (Korea); LAS (Lithuania); CINVESTAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); MST (New Zealand); PAEC (Pakistan); MSHE (Poland); NSC (Poland); FCT (Portugal); JINR (Armenia, Belarus, Georgia, Ukraine, Uzbekistan); MON (Russia); RosAtom (Russia); RAS (Russia); RFBR (Russia); MSTD (Serbia); MICINN (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); TUBITAK; TAEK (Turkey); STFC (United Kingdom); DOE (USA); NSF (USA) FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC machine. We thank the technical and administrative staff at CERN and other CMS institutes, and acknowledge support from: FMSR (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); RPF (Cyprus); MoER, SF0690030s09 and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NKTH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); NRF and WCU (Korea); LAS (Lithuania); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MST (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Armenia, Belarus, Georgia, Ukraine, Uzbekistan); MON, RosAtom, RAS and RFBR (Russia); MSTD (Serbia); MICINN and CPAN (Spain); Swiss Funding Agencies (Switzerland); NSC (Taipei); TUBITAK and TAEK (Turkey); STFC (United Kingdom); DOE and NSF (USA). NR 27 TC 3 Z9 3 U1 0 U2 64 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD NOV PY 2012 IS 11 AR 172 DI 10.1007/JHEP11(2012)172 PG 30 WC Physics, Particles & Fields SC Physics GA 056JL UT WOS:000312484500041 ER PT J AU Chatrchyan, S Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Aguilo, E Bergauer, T Dragicevic, M Ero, J Fabjan, C Friedl, M Fruhwirth, R Ghete, VM Hammer, J Hormann, N Hrubec, J Jeitler, M Kiesenhofer, W Knunz, V Krammer, M Kratschmer, I Liko, D Mikulec, I Pernicka, M Rahbaran, B Rohringer, C Rohringer, H Schofbeck, R Strauss, J Taurok, A Waltenberger, W Walzel, G Widl, E Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Bansal, M Bansal, S Cornelis, T De Wolf, EA Janssen, X Luyckx, S Mucibello, L Ochesanu, S Roland, B Rougny, R Selvaggi, M Staykova, Z Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Blekman, F Blyweert, S D'Hondt, J Suarez, RG Kalogeropoulos, A Maes, M Olbrechts, A Van Doninck, W Van Mulders, P Van Onsem, GP Villella, I Clerbaux, B De Lentdecker, G Dero, V Gay, APR Hreus, T Leonard, A Marage, PE Mohammadi, A Reis, T Thomas, L Marcken, GV Velde, CV Vanlaer, P Wang, J Adler, V Beernaert, K Cimmino, A Costantini, S Garcia, G Grunewald, M Klein, B Lellouch, J Marinov, A Mccartin, J Rios, AAO Ryckbosch, D Strobbe, N Thyssen, F Tytgat, M Verwilligen, P Walsh, S Yazgan, E Zaganidis, N Basegmez, S Bruno, G Castello, R Ceard, L Delaere, C du Pree, T Favart, D Forthomme, L Giammanco, A Hollar, J Lemaitre, V Liao, J Militaru, O Nuttens, C Pagano, D Pin, A Piotrzkowski, K Schul, N Garcia, JMV Beliy, N Caebergs, T Daubie, E Hammad, GH Alves, GA Martins, MC Damiao, DD Martins, T Pol, ME Souza, MHG Alda, WL Carvalho, W Custodio, A Da Costa, EM Martins, CD De Souza, SF Figueiredo, DM Mundim, L Nogima, H Oguri, V Da Silva, WLP Santoro, A Jorge, LS Sznajder, A Anjos, TS Bernardes, CA Dias, FA Tomei, TRFP Gregores, EM Lagana, C Marinho, F Mercadante, PG Novaes, SF Padula, SS Genchev, V Iaydjiev, P Piperov, S Rodozov, M Stoykova, S Sultanov, G Tcholakov, V Trayanov, R Vutova, M Dimitrov, A Hadjiiska, R Kozhuharov, V Litov, L Pavlov, B Petkov, P Bian, JG Chen, GM Chen, HS Jiang, CH Liang, D Liang, S Meng, X Tao, J Wang, J Wang, X Wang, Z Xiao, H Xu, M Zang, J Zhang, Z Asawatangtrakuldee, C Ban, Y Guo, Y Li, W Liu, S Mao, Y Qian, SJ Teng, H Wang, D Zhang, L Zou, W Avila, C Gomez, JP Moreno, BG Oliveros, AFO Sanabria, JC Godinovic, N Lelas, D Plestina, R Polic, D Puljak, I Antunovic, Z Kovac, M Brigljevic, V Duric, S Kadija, K Luetic, J Morovic, S Attikis, A Galanti, M Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Finger, M Finger, M Assran, Y Elgammal, S Kamel, AE Khalil, S Mahmoud, MA Radi, A Kadastik, M Muntel, M Raidal, M Rebane, L Tiko, A Eerola, P Fedi, G Voutilainen, M Harkonen, J Heikkinen, A Karimaki, V Kinnunen, R Kortelainen, MJ Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E Ungaro, D Wendland, L Banzuzi, K Karjalainen, A Korpela, A Tuuva, T Besancon, M Choudhury, S Dejardin, M Denegri, D Fabbro, B Faure, JL Ferri, F Ganjour, S Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Malcles, J Millischer, L Nayak, A Rander, J Rosowsky, A Shreyber, I Titov, M Baffioni, S Beaudette, F Benhabib, L Bianchini, L Bluj, M Broutin, C Busson, P Charlot, C Daci, N Dahms, T Dobrzynski, L de Cassagnac, RG Haguenauer, M Mine, P Mironov, C Naranjo, IN Nguyen, M Ochando, C Paganini, P Sabes, D Salerno, R Sirois, Y Veelken, C Zabi, A Agram, JL Andrea, J Bloch, D Bodin, D Brom, JM Cardaci, M Chabert, EC Collard, C Conte, E Drouhin, F Ferro, C Fontaine, JC Gele, D Goerlach, U Juillot, P Le Bihan, AC Van Hove, P Fassi, F Mercier, D Beauceron, S Beaupere, N Bondu, O Boudoul, G Chasserat, J Chierici, R Contardo, D Depasse, P El Mamouni, H Fay, J Gascon, S Gouzevitch, M Ille, B Kurca, T Lethuillier, M Mirabito, L Perries, S Sgandurra, L Sordini, V Tschudi, Y Verdier, P Viret, S Tsamalaidze, Z Anagnostou, G Autermann, C Beranek, S Edelhoff, M Feld, L Heracleous, N Hindrichs, O Jussen, R Klein, K Merz, J Ostapchuk, A Perieanu, A Raupach, F Sammet, J Schael, S Sprenger, D Weber, H Wittmer, B Zhukov, V Ata, M Caudron, J Dietz-Laursonn, E Duchardt, D Erdmann, M Fischer, R Guth, A Hebbeker, T Heidemann, C Hoepfner, K Klingebiel, D Kreuzer, P Merschmeyer, M Meyer, A Olschewski, M Papacz, P Pieta, H Reithler, H Schmitz, SA Sonnenschein, L Steggemann, J Teyssier, D Weber, M Bontenackels, M Cherepanov, V Erdogan, Y Flugge, G Geenen, H Geisler, M Ahmad, WH Hoehle, F Kargoll, B Kress, T Kuessel, Y Lingemann, J Nowack, A Perchalla, L Pooth, O Sauerland, P Stahl, A Martin, MA Behr, J Behrenhoff, W Behrens, U Bergholz, M Bethani, A Borras, K Burgmeier, A Cakir, A Calligaris, L Campbell, A Castro, E Costanza, F Dammann, D Pardos, CD Eckerlin, G Eckstein, D Flucke, G Geiser, A Glushkov, I Gunnellini, P Habib, S Hauk, J Hellwig, G Jung, H Kasemann, M Katsas, P Kleinwort, C Kluge, H Knutsson, A Kramer, M Krucker, D Kuznetsova, E Lange, W Lohmann, W Lutz, B Mankel, R Marfin, I Marienfeld, M Melzer-Pellmann, IA Meyer, AB Mnich, J Mussgiller, A Naumann-Emme, S Novgorodova, O Olzem, J Perrey, H Petrukhin, A Pitzl, D Raspereza, A Cipriano, PMR Riedl, C Ron, E Rosin, M Salfeld-Nebgen, J Schmidt, R Schoerner-Sadenius, T Sen, N Spiridonov, A Stein, M Walsh, R Wissing, C Blobel, V Draeger, J Enderle, H Erfle, J Gebbert, U Gorner, M Hermanns, T Hoing, RS Kaschube, K Kaussen, G Kirschenmann, H Klanner, R Lange, J Mura, B Nowak, F Peiffer, T Pietsch, N Rathjens, D Sander, C Schettler, H Schleper, P Schlieckau, E Schmidt, A Schroder, M Schum, T Seidel, M Sola, V Stadie, H Steinbruck, G Thomsen, J Vanelderen, L Barth, C Berger, J Boser, C Chwalek, T De Boer, W Descroix, A Dierlamm, A Feindt, M Guthoff, M Hackstein, C Hartmann, F Hauth, T Heinrich, M Held, H Hoffmann, KH Husemann, U Katkov, I Komaragiri, JR Pardo, PL Martschei, D Mueller, S Muller, T Niegel, M Nurnberg, A Oberst, O Oehler, A Ott, J Quast, G Rabbertz, K Ratnikov, F Ratnikova, N Rocker, S Schilling, FP Schott, G Simonis, HJ Stober, FM Troendle, D Ulrich, R Wagner-Kuhr, J Wayand, S Weiler, T Zeise, M Daskalakis, G Geralis, T Kesisoglou, S Kyriakis, A Loukas, D Manolakos, I Markou, A Markou, C Mavrommatis, C Ntomari, E Gouskos, L Mertzimekis, TJ Panagiotou, A Saoulidou, N Evangelou, I Foudas, C Kokkas, P Manthos, N Papadopoulos, I Patras, V Bencze, G Hajdu, C Hidas, P Horvath, D Sikler, F Veszpremi, V Vesztergombil, G Beni, N Czellar, S Molnar, J Palinkas, J Szillasi, Z Karancsi, J Raics, P Trocsanyi, ZL Ujvari, B Beri, SB Bhatnagar, V Dhingra, N Gupta, R Kaur, M Mehta, MZ Nishu, N Saini, LK Sharma, A Singh, JB Kumar, A Kumar, A Ahuja, S Bhardwaj, A Choudhary, BC Malhotra, S Naimuddin, M Ranjan, K Sharma, V Shivpuri, RK Banerjee, S Bhattacharya, S Dutta, S Comber, B Jain, S Jain, S Khurana, R Sarkar, S Sharan, M Abdulsalam, A Choudhury, RK Dutta, D Kailas, S Kumar, V Mehta, P Mohanty, AK Pant, LM Shukla, P Aziz, T Ganguly, S Guchait, M Maity, M Majumder, G Mazumdar, K Mohanty, GB Panda, B Sudhakar, K Wickramage, N Banerjee, S Dugad, S Arfaei, H Bakhshiansohi, H Etesami, SM Fahim, A Hashemi, M Hesari, H Jafari, A Khakzad, M Najafabadi, MM Mehdiabadi, SP Safarzadeh, B Zeinali, M Abbrescia, M Barbone, L Calabria, C Chhibra, SS Colaleo, A Creanza, D De Filippis, N De Palma, M Fiore, L Iaselli, G Lusito, L Maggi, G Maggi, M Marangelli, B My, S Nuzzo, S Pacifico, N Pompili, A Pugliese, G Selvaggi, G Slivestris, L Singh, G Venditti, R Zito, G Abbiendi, G Benvenuti, AC Bonacorsi, D Braibant-Giacomelli, S Brigliadori, L Capthippi, P Castro, A Cavallo, FR Cuffiani, M Dallavalle, GM Fabbri, F Fanfani, A Fasanella, D Giacomelli, P Grandi, C Guiducci, L Marcellini, S Masetti, G Meneghelli, M Montanari, A Navarria, FL Odorici, F Perrotta, A Primavera, F Rossi, AM Rovelli, T Siroli, GP Travaglini, R Albergo, S Cappello, G Chiorboli, M Costa, S Potenza, R Tricomi, A Tuve, C Barbagli, G Ciulli, V Civinini, C D'Alessandro, R Focardi, E Frosali, S Gallo, E Gonzi, S Meschini, M 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CA CMS Collaboration TI Search for electroweak production of charginos and neutralinos using leptonic final states in pp collisions at root s=7 TeV SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering ID LARGE HADRON COLLIDER; SUPERGAUGE TRANSFORMATIONS; STANDARD MODEL; SIGNALS; MSSM; TRILEPTON; PHYSICS; PIONS; LEP AB The 2011 dataset of the CMS experiment, consisting of an integrated luminosity of 4.98 fb(-1) of pp collisions at root s = 7 TeV, enables expanded searches for direct electroweak pair production of charginos and neutralinos in supersymmetric models as well as their analogs in other models of new physics. Searches sensitive to such processes, with decays to final states that contain two or more leptons, are presented. Final states with three leptons, with a same-sign lepton pair, and with an opposite-sign lepton pair in conjunction with two jets, are examined. No excesses above the standard model expectations are observed. The results are used in conjunction with previous results on four-lepton final states to exclude a range of chargino and neutralino masses from approximately 200 to 500 GeV in the context of models that assume large branching fractions of charginos and neutralinos to leptons and vector bosons. C1 [Chatrchyan, S.; Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Aguilo, E.; Bergauer, T.; Dragicevic, M.; Eroe, J.; Fabjan, C.; Friedl, M.; Fruehwirth, R.; Ghete, V. M.; Hammer, J.; Hoermann, N.; Hrubec, J.; Jeitler, M.; Kiesenhofer, W.; Knuenz, V.; Krammer, M.; Kraetschmer, I.; Liko, D.; Mikulec, I.; Pernicka, M.; Rahbaran, B.; Rohringer, C.; Rohringer, H.; Schoefbeck, R.; Strauss, J.; Taurok, A.; Waltenberger, W.; Walzel, G.; Widl, E.; Wulz, C. -E.] Inst Hochenergiephys OeAW, Vienna, Austria. [Mossolov, V.; Shumeiko, N.; Gonzalez, J. Suarez] Natl Ctr Particle & High Energy Phys, Minsk, Byelarus. 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[Anjos, T. S.; Bernardes, C. A.; Dias, F. A.; Fernandez Perez Tomei, T. R.; Gregores, E. M.; Lagana, C.; Marinho, F.; Mercadante, P. G.; Novaes, S. F.; Padula, Sandra S.] Univ Estadual Paulista, Inst Fis Teor, BR-01405 Sao Paulo, Brazil. [Genchev, V.; Iaydjiev, P.; Piperov, S.; Rodozov, M.; Stoykova, S.; Sultanov, G.; Tcholakov, V.; Trayanov, R.; Vutova, M.] Bulgarian Acad Sci, Inst Nucl Res & Nucl Energy, Sofia, Bulgaria. [Dimitrov, A.; Hadjiiska, R.; Kozhuharov, V.; Litov, L.; Pavlov, B.; Petkov, P.] Univ Sofia, BU-1126 Sofia, Bulgaria. [Bian, J. G.; Chen, G. M.; Chen, H. S.; Jiang, C. H.; Liang, D.; Liang, S.; Meng, X.; Tao, J.; Wang, J.; Wang, X.; Wang, Z.; Xiao, H.; Xu, M.; Zang, J.; Zhang, Z.] Inst High Energy Phys, Beijing 100039, Peoples R China. [Asawatangtrakuldee, C.; Ban, Y.; Li, W.; Liu, S.; Mao, Y.; Qian, S. J.; Teng, H.; Wang, D.; Zhang, L.; Zou, W.] Peking Univ, State Key Lab Nucl Phys & Tech, Beijing 100871, Peoples R China. [Avila, C.; Gomez, J. P.; Gomez Moreno, B.; Osorio Oliveros, A. F.; Sanabria, J. C.] Univ Los Andes, Bogota, Colombia. [Godinovic, N.; Lelas, D.; Plestina, R.; Polic, D.; Puljak, I.] Tech Univ Split, Split, Croatia. [Antunovic, Z.; Kovac, M.] Univ Split, Split, Croatia. [Brigljevic, V.; Duric, S.; Kadija, K.; Luetic, J.; Morovic, S.] Rudjer Boskovic Inst, Zagreb, Croatia. [Attikis, A.; Galanti, M.; Mavromanolakis, G.; Mousa, J.; Nicolaou, C.; Ptochos, F.; Razis, P. A.] Univ Cyprus, Nicosia, Cyprus. [Finger, M.; Finger, M., Jr.] Charles Univ Prague, Prague, Czech Republic. [Assran, Y.; Elgammal, S.; Kamel, A. Ellithi; Khalil, S.; Mahmoud, M. A.; Radi, A.] Acad Sci Res & Technol Arab Republ Egypt, Egyptian Network High Energy Phys, Cairo, Egypt. [Kadastik, M.; Muntel, M.; Raidal, M.; Rebane, L.; Tiko, A.] NICPB, Tallinn, Estonia. [Eerola, P.; Fedi, G.; Voutilainen, M.] Univ Helsinki, Dept Phys, Helsinki, Finland. [Harkonen, J.; Heikkinen, A.; Karimaki, V.; Kinnunen, R.; Kortelainen, M. J.; Lampen, T.; Lassila-Perini, K.; Lehti, S.; Linden, T.; Luukka, P.; Maenpaa, T.; Peltola, T.; Tuominen, E.; Tuominiemi, J.; Tuovinen, E.; Ungaro, D.; Wendland, L.] Helsinki Inst Phys, Helsinki, Finland. [Banzuzi, K.; Karjalainen, A.; Korpela, A.; Tuuva, T.] Lappeenranta Univ Technol, Lappeenranta, Finland. [Maenpaa, T.; Besancon, M.; Choudhury, S.; Dejardin, M.; Denegri, D.; Fabbro, B.; Faure, J. L.; Ferri, F.; Ganjour, S.; Givernaud, A.; Gras, P.; de Monchenault, G. Hamel; Jarry, P.; Locci, E.; Malcles, J.; Millischer, L.; Nayak, A.; Rander, J.; Rosowsky, A.; Shreyber, I.; Titov, M.] CEA Saclay, IRFU, DSM, F-91191 Gif Sur Yvette, France. [Plestina, R.; Baffioni, S.; Beaudette, F.; Benhabib, L.; Bianchini, L.; Bluj, M.; Broutin, C.; Busson, P.; Charlot, C.; Daci, N.; Dahms, T.; Dobrzynski, L.; de Cassagnac, R. Granier; Haguenauer, M.; Mine, P.; Mironov, C.; Naranjo, I. N.; Nguyen, M.; Ochando, C.; Paganini, P.; Sabes, D.; Salerno, R.; Sirois, Y.; Veelken, C.; Zabi, A.; Bernet, C.] Ecole Polytech, CNRS, IN2P3, Lab Leprince Ringuet, F-91128 Palaiseau, France. [Agram, J. -L.; Andrea, J.; Bloch, D.; Bodin, D.; Brom, J. -M.; Cardaci, M.; Chabert, E. C.; Collard, C.; Conte, E.; Drouhin, F.; Ferro, C.; Fontaine, J. -C.; Gele, D.; Goerlach, U.; Juillot, P.; Le Bihan, A. -C.; Van Hove, P.] Univ Haute Alsace Mulhouse, Univ Strasbourg, Inst Pluridisciplinaire Hubert Curien, CNRS,IN2P3, Strasbourg, France. [Fassi, F.; Mercier, D.] CNRS, IN2P3, Ctr Calcul Inst Natl Phys Nucl & Phys Particules, Villeurbanne, France. [Beauceron, S.; Beaupere, N.; Bondu, O.; Boudoul, G.; Chasserat, J.; Chierici, R.; Contardo, D.; Depasse, P.; El Mamouni, H.; Fay, J.; Gascon, S.; Gouzevitch, M.; Ille, B.; Kurca, T.; Lethuillier, M.; Mirabito, L.; Perries, S.; Sgandurra, L.; Sordini, V.; Tschudi, Y.; Verdier, P.; Viret, S.] Univ Lyon 1, CNRS, IN2P3, Inst Phys Nucl Lyon, F-69622 Villeurbanne, France. [Tsamalaidze, Z.] Tbilisi State Univ, Inst High Energy Phys & Informatizat, GE-380086 Tbilisi, Rep of Georgia. [Anagnostou, G.; Autermann, C.; Beranek, S.; Edelhoff, M.; Feld, L.; Heracleous, N.; Hindrichs, O.; Jussen, R.; Klein, K.; Merz, J.; Ostapchuk, A.; Perieanu, A.; Raupach, F.; Sammet, J.; Schael, S.; Sprenger, D.; Weber, H.; Wittmer, B.; Zhukov, V.] Rhein Westfal TH Aachen, Inst Phys 1, Aachen, Germany. [Ata, M.; Caudron, J.; Dietz-Laursonn, E.; Duchardt, D.; Erdmann, M.; Fischer, R.; Gueth, A.; Hebbeker, T.; Heidemann, C.; Hoepfner, K.; Klingebiel, D.; Kreuzer, P.; Merschmeyer, M.; Meyer, A.; Olschewski, M.; Papacz, P.; Pieta, H.; Reithler, H.; Schmitz, S. A.; Sonnenschein, L.; Steggemann, J.; Teyssier, D.; Weber, M.] Rhein Westfal TH Aachen, Phys Inst 3A, Aachen, Germany. [Bontenackels, M.; Cherepanov, V.; Erdogan, Y.; Fluegge, G.; Geenen, H.; Geisler, M.; Ahmad, W. Haj; Hoehle, F.; Kargoll, B.; Kress, T.; Kuessel, Y.; Lingemann, J.; Nowack, A.; Perchalla, L.; Pooth, O.; Sauerland, P.; Stahl, A.] Rhein Westfal TH Aachen, Phys Inst 3B, Aachen, Germany. [Martin, M. Aldaya; Behr, J.; Behrenhoff, W.; Behrens, U.; Bergholz, M.; Bethani, A.; Borras, K.; Burgmeier, A.; Cakir, A.; Calligaris, L.; Campbell, A.; Castro, E.; Costanza, F.; Dammann, D.; Pardos, C. Diez; Eckerlin, G.; Eckstein, D.; Flucke, G.; Geiser, A.; Glushkov, I.; Gunnellini, P.; Habib, S.; Hauk, J.; Hellwig, G.; Jung, H.; Kasemann, M.; Katsas, P.; Kleinwort, C.; Kluge, H.; Knutsson, A.; Kraemer, M.; Kruecker, D.; Kuznetsova, E.; Lange, W.; Lohmann, W.; Lutz, B.; Mankel, R.; Marfin, I.; Marienfeld, M.; Melzer-Pellmann, I. -A.; Meyer, A. B.; Mnich, J.; Mussgiller, A.; Naumann-Emme, S.; Novgorodova, O.; Olzem, J.; Perrey, H.; Petrukhin, A.; Pitzl, D.; Raspereza, A.; Cipriano, P. M. Ribeiro; Riedl, C.; Ron, E.; Rosin, M.; Salfeld-Nebgen, J.; Schmidt, R.; Schoerner-Sadenius, T.; Sen, N.; Spiridonov, A.; Stein, M.; Walsh, R.; Wissing, C.] DESY, Hamburg, Germany. [Blobel, V.; Draeger, J.; Enderle, H.; Erfle, J.; Gebbert, U.; Goerner, M.; Hermanns, T.; Hoeing, R. S.; Kaschube, K.; Kaussen, G.; Kirschenmann, H.; Klanner, R.; Lange, J.; Mura, B.; Nowak, F.; Peiffer, T.; Pietsch, N.; Rathjens, D.; Sander, C.; Schettler, H.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Schroeder, M.; Schum, T.; Seidel, M.; Sola, V.; Stadie, H.; Steinbrueck, G.; Thomsen, J.; Vanelderen, L.] Univ Hamburg, Hamburg, Germany. [Barth, C.; Berger, J.; Boeser, C.; Chwalek, T.; De Boer, W.; Descroix, A.; Dierlamm, A.; Feindt, M.; Guthoff, M.; Hackstein, C.; Hartmann, F.; Hauth, T.; Heinrich, M.; Held, H.; Hoffmann, K. H.; Husemann, U.; Katkov, I.; Komaragiri, J. R.; Pardo, P. Lobelle; Martschei, D.; Mueller, S.; Mueller, Th.; Niegel, M.; Nuernberg, A.; Oberst, O.; Oehler, A.; Ott, J.; Quast, G.; Rabbertz, K.; Ratnikov, F.; Ratnikova, N.; Roecker, S.; Schilling, F. -P.; Schott, G.; Simonis, H. J.; Stober, F. M.; Troendle, D.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weiler, T.; Zeise, M.] Univ Karlsruhe, Inst Expt Kernphys, D-7500 Karlsruhe, Germany. [Daskalakis, G.; Geralis, T.; Kesisoglou, S.; Kyriakis, A.; Loukas, D.; Manolakos, I.; Markou, A.; Markou, C.; Mavrommatis, C.; Ntomari, E.] Inst Nucl Phys Demokritos, Aghia Paraskevi, Greece. [Gouskos, L.; Mertzimekis, T. J.; Panagiotou, A.; Saoulidou, N.; Sphicas, P.] Univ Athens, Athens, Greece. [Evangelou, I.; Foudas, C.; Kokkas, P.; Manthos, N.; Papadopoulos, I.; Patras, V.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombil, G.; Krajczar, K.] KFKI Res Inst Particle & Nucl Phys, Budapest, Hungary. [Horvath, D.; Beni, N.; Czellar, S.; Molnar, J.; Palinkas, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Karancsi, J.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, H-4012 Debrecen, Hungary. [Beri, S. B.; Bhatnagar, V.; Dhingra, N.; Gupta, R.; Kaur, M.; Mehta, M. Z.; Nishu, N.; Saini, L. K.; Sharma, A.; Singh, J. B.] Panjab Univ, Chandigarh 160014, India. [Kumar, Ashok; Kumar, Arun; Ahuja, S.; Bhardwaj, A.; Choudhary, B. C.; Malhotra, S.; Naimuddin, M.; Ranjan, K.; Sharma, V.; Shivpuri, R. K.] Univ Delhi, Delhi 110007, India. [Banerjee, S.; Bhattacharya, S.; Dutta, S.; Comber, B.; Jain, Sa.; Jain, Sh.; Khurana, R.; Sarkar, S.; Sharan, M.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Choudhury, R. K.; Dutta, D.; Kailas, S.; Kumar, V.; Mehta, P.; Mohanty, A. K.; Pant, L. M.; Shukla, P.] Bhabha Atom Res Ctr, Bombay 400085, Maharashtra, India. [Aziz, T.; Ganguly, S.; Guchait, M.; Maity, M.; Majumder, G.; Mazumdar, K.; Mohanty, G. B.; Panda, B.; Sudhakar, K.; Wickramage, N.] Tata Inst Fundamental Res EHEP, Bombay, Maharashtra, India. [Guchait, M.; Banerjee, S.; Dugad, S.] Tata Inst Fundamental Res HECR, Bombay, Maharashtra, India. [Arfaei, H.; Bakhshiansohi, H.; Etesami, S. M.; Fahim, A.; Hashemi, M.; Hesari, H.; Jafari, A.; Khakzad, M.; Najafabadi, M. Mohammadi; Mehdiabadi, S. Paktinat; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; Colaleo, A.; Creanza, D.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Lusito, L.; Maggi, G.; Maggi, M.; Marangelli, B.; My, S.; Nuzzo, S.; Pacifico, N.; Pompili, A.; Pugliese, G.; Selvaggi, G.; Slivestris, L.; Singh, G.; Venditti, R.; Zito, G.] INFN Sez Bari, Bari, Italy. [Abbrescia, M.; Barbone, L.; Calabria, C.; Chhibra, S. S.; De Palma, M.; Lusito, L.; Marangelli, B.; Nuzzo, S.; Pacifico, N.; Pompili, A.; Selvaggi, G.; Singh, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Capthippi, P.; Castro, A.; Cavallo, F. R.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Meneghelli, M.; Montanari, A.; Navarria, F. L.; Odorici, F.; Perrotta, A.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Travaglini, R.] INFN Sez Bologna, Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Capthippi, P.; Castro, A.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Meneghelli, M.; Navarria, F. L.; Primavera, F.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] INFN Sez Catania, Catania, Italy. [Albergo, S.; Cappello, G.; Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gallo, E.; Gonzi, S.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.] INFN Sez Firenze, Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Frosali, S.; Gonzi, S.; Tropiano, A.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Colafranceschi, S.; Fabbri, F.; Piccolo, D.] INFN Lab Nazl Frascati, Frascati, Italy. [Fabbricatore, P.; Musenich, R.; Tosi, S.] INFN Sez Genova, Genoa, Italy. [Tosi, S.] Univ Genoa, Genoa, Italy. [Benaglia, A.; De Guio, F.; Di Matteo, L.; Fiorendi, S.; Gennai, S.; Ghezzi, A.; Malvezzi, S.; Manzoni, R. A.; Martelli, A.; Massironi, A.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; Sala, S.; de Fatis, T. Tabarelli] INFN Sez Milano Bicocca, Milan, Italy. [Benaglia, A.; De Guio, F.; Di Matteo, L.; Fiorendi, S.; Ghezzi, A.; Manzoni, R. A.; Martelli, A.; Massironi, A.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Montoya, C. A. Carrillo; Cavallo, N.; De Cosa, A.; Dogangun, O.; Fabozzi, F.; Iorio, A. O. M.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.] INFN Sez Napoli, Naples, Italy. [De Cosa, A.; Dogangun, O.; Iorio, A. O. M.; Merola, M.] Univ Naples Federico II, Naples, Italy. [Azzi, P.; Bacchetta, N.; Bellan, P.; Bisello, D.; Branca, A.; Carlin, R.; Checchia, P.; Dorigo, T.; Dosselli, U.; Gasparini, F.; Gasparini, U.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Lazzizzera, I.; Margoni, M.; Meneguzzo, A. T.; Nespolo, M.; Pazzini, J.; Ronchese, P.; Simonetto, F.; Torassa, E.; Vanini, S.; Zotto, P.; Zumerle, G.] INFN Sez Padova, Padua, Italy. [Bellan, P.; Bisello, D.; Branca, A.; Carlin, R.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Ronchese, P.; Simonetto, F.; Vanini, S.; Zotto, P.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.; Lazzizzera, I.] Univ Trento Trento, Padua, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Torre, P.; Vitulo, P.] INFN Sez Pavia, Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Torre, P.; Vitulo, P.] Univ Pavia, I-27100 Pavia, Italy. [Pioppi, M.] Univ Perugia, INFN Sez Perugia, I-06100 Perugia, Italy. [Azzurri, P.; Bagliesi, G.; Boccali, T.; Broccolo, G.; Castaldi, R.; D'Agnolo, R. T.; Dell'Orso, R.; Fiori, F.; Foa, L.; Giassi, A.; Kraan, A.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. C.] INFN Sez Pisa, Pisa, Italy. [Fiori, F.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Azzurri, P.; Broccolo, G.; D'Agnolo, R. T.; Foa, L.; Ligabue, F.] Scuola Normale Super Pisa, Pisa, Italy. [Rovelli, C.] Univ Rome, INFN Sez Roma, Rome, Italy. [Colafranceschi, S.] Univ Rome, Fac Ingn, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Biino, C.; Cartiglia, N.; Costa, M.; Demaria, N.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Musich, M.; Obertino, M. M.; Pastrone, N.; Pelliccioni, M.; Potenza, A.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Pereira, A. Vilela] INFN Sez Torino, Turin, Italy. [Amapane, N.; Argiro, S.; Costa, M.; Migliore, E.; Monaco, V.; Potenza, A.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Obertino, M. M.; Ruspa, M.] Univ Piemonte Orientale Novara, Turin, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; Marone, M.; Montanino, D.; Penzo, A.; Schizzi, A.] INFN Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; Marone, M.; Montanino, D.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Heo, S. C.; Kim, T. Y.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Chang, S.; Kim, D. H.; Kim, G. N.; Kong, D. J.; Park, H.; Ro, S. R.; Son, D. C.; Son, T.; Kamon, T.] Kyungpook Natl Univ, Taegu, South Korea. [Kim, J. Y.; Kim, Zero J.; Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, T. J.; Lee, K. S.; Moon, D. H.; Park, S. K.] Korea Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Park, C.; Park, I. C.; Park, S.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Cho, Y.; Choi, Y.; Choi, Y. K.; Goh, J.; Kim, M. S.; Kwon, E.; Lee, B.; Lee, J.; Lee, S.; Seo, H.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Bilinskas, M. J.; Grigelionis, I.; Janulis, M.; Juodagalvis, A.] Vilnius State Univ, Vilnius, Lithuania. [Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Lopez-Fernandez, R.; Magana Villalba, R.; Martinez-Ortega, J.; Sanchez-Hernandez, A.; Villasenor-Cendejas, L. M.] Ctr Invest & Estudios Avanzados IPN, Mexico City, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Casimiro Linares, E.; Morelos Pineda, A.; Reyes-Santos, M. A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Bell, A. J.; Butler, P. H.; Doesburg, R.; Reucroft, S.; Silverwood, H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Ansari, M. H.; Asghar, M. I.; Hoorani, H. R.; Khalid, S.; Khan, W. A.; Khurshid, T.; Qazi, S.; Shah, M. A.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Boimska, B.; Frueboes, T.; Gokieli, R.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Wrochna, G.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Cwiok, M.; Dominik, W.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Almeida, N.; Bargassa, P.; David, A.; Faccioli, P.; Ferreira Parracho, P. C.; Gallinaro, M.; Seixas, J.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Tsamalaidze, Z.; Belotelov, I.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Kozlov, G.; Laney, A.; Malakhov, A.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Smirnov, V.; Volodko, A.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Evstyukhin, S.; Golovtsov, V.; Ivanov, Y.; Kim, V.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.; Vorobyev, An.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Kirsanov, M.; Krasnikov, N.; Matveev, V.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow, Russia. [Epshteyn, V.; Erofeeva, M.; Gavrilov, V.; Kossov, M.; Lychkovskaya, N.; Popov, V.; Safronov, G.; Semenov, S.; Stolin, V.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Zhukov, V.; Katkov, I.; Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Markina, A.; Obraztsov, S.; Perfilov, M.; Petrushanko, S.; Popov, A.; Sarychevat, L.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Grishin, V.; Kachanov, V.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade 11001, Serbia. [Adzic, P.; Djordjevic, M.; Ekmedzic, M.; Krpic, D.; Milosevic, J.; Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Aguilar-Benitez, M.; Alcaraz Maestre, J.; Arce, P.; Battilana, C.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Ferrando, A.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Merino, G.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.; Willmott, C.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain. [Albajar, C.; Codispoti, G.; de Troconiz, J. F.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Lloret Iglesias, L.; Piedra Gomez, J.] Univ Oviedo, Oviedo, Spain. [Brochero Cifuentes, J. A.; Cabrillo, I. J.; Calderon, A.; Chuang, S. H.; Duarte Campderros, J.; Felcini, M.; Fernandez, M.; Gomez, G.; Gonzalez Sanchez, J.; Graziano, A.; Jorda, C.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] CSIC Univ Cantabria, Inst Fis Cantabria IFCA, Santander, Spain. [Genchev, V.; Iaydjiev, P.; Puljak, I.; Chierici, R.; Lingemann, J.; Guthoff, M.; Hauth, T.; Mohanty, A. K.; Calabria, C.; De Filippis, N.; Fasanella, D.; Meneghelli, M.; Di Matteo, L.; Gennai, S.; Massironi, A.; De Cosa, A.; Paolucci, P.; Bacchetta, N.; Branca, A.; Nespolo, M.; D'Agnolo, R. T.; Fiori, F.; Squillacioti, P.; Grassi, M.; Meridiani, P.; Mariotti, C.; Musich, M.; Marone, M.; Montanino, D.; Grishin, V.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benitez, J. F.; Bernet, C.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Christiansen, T.; Perez, J. A. Coarasa; D'Enterria, D.; Dabrowski, A.; De Roeck, A.; Di Guida, S.; Dobson, M.; Dupont-Sagorin, N.; Elliott-Peisert, A.; Frisch, B.; Funk, W.; Georgiou, G.; Giffels, M.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Giunta, M.; Glege, F.; Garrido, R. Gomez-Reino; Govoni, P.; Gowdy, S.; Guida, R.; Hansen, M.; Harris, P.; Hartl, C.; Harvey, J.; Hegner, B.; Hinzmann, A.; Innocente, V.; Janot, P.; Kaadze, K.; Karavakis, E.; Kousouris, K.; Lecoq, P.; Lee, Y. -J.; Lenzi, P.; Lourenco, C.; Magini, N.; Maeki, T.; Malberti, M.; Malgeri, L.; Mannelli, M.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moser, R.; Mozer, M. U.; Mulders, M.; Musella, P.; Nesvold, E.; Orimoto, T.; Orsini, L.; Cortezon, E. Palencia; Perez, E.; Perrozzi, L.; Petrilli, A.; Pfeiffer, A.; Pierini, M.; Pimiae, M.; Piparo, D.; Polese, G.; Quertenmont, L.; Racz, A.; Reece, W.; Antunes, J. Rodrigues; Rolandi, G.; Rovelli, C.; Rovere, M.; Sakulin, H.; Santanastasio, F.; Schaefer, C.; Schwick, C.; Segoni, I.; Sekmen, S.; Sharma, A.; Siegrist, P.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Tsirou, A.; Veres, G. I.; Vlimant, J. R.; Woehri, H. K.; Worm, S. D.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Gabathuler, K.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Koenig, S.; Kotlinski, D.; Langenegger, U.; Meier, F.; Renker, D.; Rohe, T.; Sibille, J.; Naegeli, C.] Paul Scherrer Inst, Villigen, Switzerland. [Baeni, L.; Bortignon, P.; Buchmann, M. A.; Casal, B.; Chanon, N.; Deisher, A.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eugster, J.; Freudenreich, K.; Grab, C.; Hits, D.; Lecomte, P.; Lustermann, W.; Marini, A. C.; del Arbol, P. Martinez Ruiz; Mohr, N.; Moortgat, F.; Naegeli, C.; Nef, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pape, L.; Pauss, F.; Peruzzi, M.; Ronga, F. J.; Rossini, M.; Sala, L.; Sanchez, A. K.; Starodumov, A.; Stieger, B.; Takahashi, M.; Tauscher, L.; Thea, A.; Theofilatos, K.; Treille, D.; Urscheler, C.; Wallny, R.; Weber, H. A.; Wehrli, L.] Swiss Fed Inst Technol, Inst Particle Phys, Zurich, Switzerland. [Amsler, C.; Chiochia, V.; De Visscher, S.; Favaro, C.; Rikova, M. Ivova; Mejias, B. Millan; Otiougova, P.; Robmann, P.; Snoek, H.; Tupputi, S.; Verzetti, M.] Univ Zurich, Zurich, Switzerland. [Chang, Y. H.; Chen, K. H.; Kuo, C. M.; Li, S. W.; Lin, W.; Liu, Z. K.; Lu, Y. J.; Mekterovic, D.; Singh, A. P.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli, Taiwan. [Bartalini, P.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Dietz, C.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Kao, K. Y.; Lei, Y. J.; Lu, R. -S.; Majumder, D.; Petrakou, E.; Shi, X.; Shiu, J. G.; Tzeng, Y. M.; Wan, X.; Wang, M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Srimanobhas, N.] Chulalongkorn Univ, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Karaman, T.; Karapinar, G.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Sogut, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Vergili, L. N.; Vergili, M.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Aliev, T.; Bilin, B.; Bilmis, S.; Deniz, M.; Gamsizkan, H.; Guler, A. M.; Ocalan, K.; Ozpineci, A.; Serin, M.; Sever, R.; Surat, U. E.; Yalvac, M.; Yildirim, E.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Isildak, B.; Kaya, M.; Kaya, O.; Ozkorucuklu, S.; Sonmez, N.] Bogazici Univ, Istanbul, Turkey. [Cankocak, K.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Levchuk, L.] Kharkov Phys & Technol Inst, Natl Sci Ctr, UA-310108 Kharkov, Ukraine. [Bostock, F.; Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Frazier, R.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Kreczko, L.; Metson, S.; Newbold, D. M.; Nirunpong, K.; Poll, A.; Senkin, S.; Smith, V. J.; Williams, T.] Univ Bristol, Bristol, Avon, England. [Worm, S. D.; Newbold, D. M.; Basso, L.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Jackson, J.; Kennedy, B. W.; Olaiya, E.; Petyt, D.; Radburn-Smith, B. C.; Shepherd-Themistocleous, C. H.; Tomalin, I. R.; Womersley, W. J.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Bainbridge, R.; Ball, G.; Beuselinck, R.; Buchmuller, O.; Colling, D.; Cripps, N.; Cutajar, M.; Dauncey, P.; Davies, G.; Della Negra, M.; Ferguson, W.; Fulcher, J.; Futyan, D.; Gilbert, A.; Bryer, A. Guneratne; Hall, G.; Hatherell, Z.; Hays, J.; Iles, G.; Jarvis, M.; Karapostoli, G.; Lyons, L.; Magnan, A. -M.; Marrouche, J.; Mathias, B.; Nandi, R.; Nash, J.; Nikitenko, A.; Papageorgiou, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Pioppi, M.; Raymond, D. M.; Rogerson, S.; Rose, A.; Ryan, M. J.; Seez, C.; Sharp, P.; Sparrow, A.; Stoye, M.; Tapper, A.; Acosta, M. Vazquez; Virdee, T.; Wakefield, S.; Wardle, N.; Whyntie, T.] Univ London Imperial Coll Sci Technol & Med, London, England. [Chadwick, M.; Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Martin, W.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Hatakeyama, K.; Liu, H.; Scarborough, T.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Heister, A.; John, J. St.; Lawson, P.; Lazic, D.; Rohlf, J.; Sperka, D.; Sulak, L.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Bhattacharya, S.; Cutts, D.; Demiragli, Z.; Ferapontov, A.; Heintz, U.; Jabeen, S.; Kukartsev, G.; Laird, E.; Landsberg, G.; Luk, M.; Narain, M.; Nguyen, D.; Segala, M.; Sinthuprasith, T.; Speer, T.; Tsang, K. V.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Dolen, J.; Erbacher, R.; Gardner, M.; Houtz, R.; Ko, W.; Kopecky, A.; Lander, R.; Mall, O.; Miceli, T.; Pellett, D.; Ricci-tam, F.; Rutherford, B.; Searle, M.; Smith, J.; Squires, M.; Tripathi, M.; Sierra, R. Vasquez; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Felcini, M.; Andreev, V.; Cline, D.; Cousins, R.; Duris, J.; Erhan, S.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Jarvis, C.; Plager, C.; Rakness, G.; Schlein, P.; Traczyk, P.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Babb, J.; Clare, R.; Dinardo, M. E.; Ellison, J.; Gary, J. W.; Giordano, F.; Hanson, G.; Jeng, G. Y.; Liu, H.; Long, O. R.; Luthra, A.; Nguyen, H.; Paramesvaran, S.; Sturdy, J.; Sumowidagdo, S.; Wilken, R.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Andrews, W.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; Evans, D.; Golf, F.; Holzner, A.; Kelley, R.; Lebourgeois, M.; Letts, J.; Macneill, I.; Mangano, B.; Padhi, S.; Palmer, C.; Petrucciani, G.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Sudano, E.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Wuerthwein, F.; Yagil, A.; Yoo, J.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bellan, R.; Campagnari, C.; D'Alfonso, M.; Danielson, T.; Flowers, K.; Geffert, P.; Incandela, J.; Justus, C.; Kalavase, P.; Koay, S. A.; Kovalskyi, D.; Krutelyov, V.; Lowette, S.; Mccoll, N.; Pavlunin, V.; Rebassoo, F.; Ribnik, J.; Richman, J.; Rossin, R.; Stuart, D.; To, W.; West, C.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dias, F. A.; Dubinin, M.; Apresyan, A.; Bornheim, A.; Chen, Y.; Di Marco, E.; Duarte, J.; Gataullin, M.; Ma, Y.; Mott, A.; Newman, H. B.; Rogan, C.; Spiropulu, M.; Timciuc, V.; Veverka, J.; Wilkinson, R.; Xie, S.; Yang, Y.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Akgun, B.; Azzolini, V.; Calamba, A.; Carroll, R.; Ferguson, T.; Iiyama, Y.; Jang, D. W.; Liu, Y. F.; Paulini, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Drell, B. R.; Ford, W. T.; Gaz, A.; Lopez, E. Luiggi; Smith, J. G.; Stenson, K.; Ulmer, K. A.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Eggert, N.; Gibbons, L. K.; Heltsley, B.; Khukhunaishvili, A.; Kreis, B.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Ryd, A.; Salvati, E.; Sun, W.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Vaughan, J.; Weng, Y.; Winstrom, L.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bloch, I.; Burkett, K.; Butler, J. N.; Chetluru, V.; Cheung, H. W. K.; Chlebana, F.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gao, Y.; Green, D.; Gutsche, O.; Hanlon, J.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Kilminster, B.; Klima, B.; Kunori, S.; Kwan, S.; Leonidopoulos, C.; Linacre, J.; Lincoln, D.; Lipton, R.; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Maruyama, S.; Mason, D.; McBride, P.; Mishra, K.; Mrenna, S.; Musienko, Y.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Sexton-Kennedy, E.; Sharma, S.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vidal, R.; Whitmore, J.; Wu, W.; Yang, F.; Yumiceva, F.; Yun, J. C.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bourilkov, D.; Chen, M.; Cheng, T.; Das, S.; De Gruttola, M.; Di Giovanni, G. P.; Dobur, D.; Drozdetskiy, A.; Field, R. D.; Fisher, M.; Fu, Y.; Furic, I. K.; Gartner, J.; Hugon, J.; Kim, B.; Konigsberg, J.; Korytov, A.; Kropivnitskaya, A.; Kypreos, T.; Low, J. F.; Matchev, K.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Park, M.; Remington, R.; Rinkevicius, A.; Sellers, P.; Skhirtladze, N.; Snowball, M.; Yelton, J.; Zakaria, M.] Univ Florida, Gainesville, FL USA. [Gaultney, V.; Hewamanage, S.; Lebolo, L. M.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Adams, T.; Askew, A.; Bochenek, J.; Chen, J.; Diamond, B.; Gleyzer, S. V.; Haas, J.; Hagopian, S.; Hagopian, V.; Jenkins, M.; Johnson, K. F.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Dorney, B.; Hohlmann, M.; Kalakhety, H.; Vodopiyanov, I.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Anghel, I. M.; Apanasevich, L.; Bai, Y.; Bazterra, V. E.; Betts, R. R.; Bucinskaite, I.; Callner, J.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Khalatyan, S.; Lacroix, F.; Malek, M.; O'Brien, C.; Silkworth, C.; Strom, D.; Turner, P.; Varelas, N.] Univ Illinois Chicago UIC, Chicago, IL USA. [Ozturk, S.; Akgun, U.; Albayrak, E. A.; Bilki, B.; Clarida, W.; Duru, F.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Newsom, C. R.; Norbeck, E.; Onel, Y.; Ozok, F.; Sen, S.; Tan, P.; Tiras, E.; Wetzel, J.; Yetkin, T.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Bolognesi, S.; Fehling, D.; Giurgiu, G.; Gritsan, A. V.; Guo, Z. J.; Hu, G.; Maksimovic, P.; Rappoccio, S.; Swartz, M.; Whitbeck, A.] Johns Hopkins Univ, Baltimore, MD USA. [Sibille, J.; Baringer, P.; Bean, A.; Benelli, G.; Iii, R. P. Kenny; Murray, M.; Noonan, D.; Sanders, S.; Stringer, R.; Tinti, G.; Wood, J. S.; Zhukova, V.] Univ Kansas, Lawrence, KS 66045 USA. [Barfuss, A. F.; Bolton, T.; Chakaberia, I.; Ivanov, A.; Khalil, S.; Makouski, M.; Maravin, Y.; Shrestha, S.; Svintradze, I.] Kansas State Univ, Manhattan, KS 66506 USA. [Gronberg, J.; Lange, D.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Baden, A.; Boutemeur, M.; Calvert, B.; Eno, S. C.; Gomez, J. A.; Hadley, N. J.; Kellogg, R. G.; Kim, M.; Kolberg, T.; Lu, Y.; Marionneau, M.; Mignerey, A. C.; Pedro, K.; Peterman, A.; Skuja, A.; Temple, J.; Tonjes, M. B.; Tonwar, S. C.; Twedt, E.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Bauer, G.; Bendavid, J.; Busza, W.; Butz, E.; Cali, I. A.; Chan, M.; Dutta, V.; Ceballos, G. Gomez; Goncharov, M.; Hahn, K. A.; Kim, Y.; Klute, M.; Krajczar, K.; Luckey, P. D.; Ma, T.; Nahn, S.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Rudolph, M.; Stephans, G. S. F.; Stoeckli, F.; Sumorok, K.; Sung, K.; Velicanu, D.; Wenger, E. A.; Wolf, R.; Wyslouch, B.; Yang, M.; Yilmaz, Y.; Yoon, A. S.; Zanetti, M.] MIT, Cambridge, MA 02139 USA. [Cooper, S. I.; Dahmes, B.; De Benedetti, A.; Franzoni, G.; Gude, A.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Mans, J.; Pastika, N.; Rusack, R.; Sasseville, M.; Singovsky, A.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Cremaldi, L. M.; Kroeger, R.; Perera, L.; Rahmat, R.; Sanders, D. A.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Butt, J.; Claes, D. R.; Dominguez, A.; Eads, M.; Keller, J.; Kravchenko, I.; Lazo-Flores, J.; Malbouisson, H.; Malik, S.; Snow, G. R.] Univ Nebraska Lincoln, Lincoln, NE USA. [Godshalk, A.; Iashvili, I.; Jain, S.; Kharchilava, A.; Kumar, A.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Haley, J.; Nash, D.; Trocino, D.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Anastassov, A.; Kubik, A.; Mucia, N.; Odell, N.; Ofierzynski, R. A.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Velasco, M.; Won, S.] Northwestern Univ, Evanston, IL USA. [Antonelli, L.; Berry, D.; Brinkerhoff, A.; Chan, K. M.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kolb, J.; Lannon, K.; Luo, W.; Lynch, S.; Marinelli, N.; Morse, D. M.; Pearson, T.; Planer, M.; Ruchti, R.; Slaunwhite, J.; Valls, N.; Wayne, M.; Wolf, M.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Bylsma, B.; Durkin, L. S.; Hill, C.; Hughes, R.; Kotov, K.; Ling, T. Y.; Puigh, D.; Rodenburg, M.; Vuosalo, C.; Williams, G.; Winer, B. L.] Ohio State Univ, Columbus, OH 43210 USA. [Adam, N.; Berry, E.; Elmer, P.; Gerbaudo, D.; Halyo, V.; Hebda, P.; Hegeman, J.; Hunt, A.; Jindal, P.; Pegna, D. Lopes; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Piroue, P.; Quan, X.; Raval, A.; Safdi, B.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Brownson, E.; Lopez, A.; Mendez, H.; Vargas, J. E. Ramirez] Univ Puerto Rico, Mayaguez, PR USA. [Alagoz, E.; Barnes, V. E.; Benedetti, D.; Bolla, G.; Bortoletto, D.; De Mattia, M.; Everett, A.; Hu, Z.; Jones, M.; Koybasi, O.; Kress, M.; Laasanen, A. T.; Leonardo, N.; Maroussov, V.; Merkel, P.; Miller, D. H.; Neumeister, N.; Shipsey, I.; Silvers, D.; Svyatkovskiy, A.; Marono, M. Vidal; Yoo, H. D.; Zablocki, J.; Zheng, Y.] Purdue Univ, W Lafayette, IN 47907 USA. [Guragain, S.; Parashar, N.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Boulahouache, C.; Ecklund, K. M.; Geurts, F. J. M.; Li, W.; Padley, B. P.; Redjimi, R.; Roberts, J.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; Chung, Y. S.; Covarelli, R.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Hard, A.; Miner, D. C.; Vishnevskiy, D.; Zielinski, M.] Univ Rochester, Rochester, NY 14627 USA. [Bhatti, A.; Ciesielski, R.; Demortier, L.; Goulianos, K.; Lungu, G.; Malik, S.; Mesropian, C.] Rockefeller Univ, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Lath, A.; Panwalkar, S.; Park, M.; Patel, R.; Rekovic, V.; Robles, J.; Rose, K.; Salur, S.; Schnetzer, S.; Seitz, C.; Somalwar, S.; Stone, R.; Thomas, S.] Rutgers State Univ, Piscataway, NJ USA. [Cerizza, G.; Hollingsworth, M.; Spanier, S.; Yang, Z. C.; York, A.] Univ Tennessee, Knoxville, TN USA. 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RI Calderon, Alicia/K-3658-2014; de la Cruz, Begona/K-7552-2014; Scodellaro, Luca/K-9091-2014; Josa, Isabel/K-5184-2014; Calvo Alamillo, Enrique/L-1203-2014; Paulini, Manfred/N-7794-2014; Vogel, Helmut/N-8882-2014; Marinho, Franciole/N-8101-2014; Ferguson, Thomas/O-3444-2014; Benussi, Luigi/O-9684-2014; Grandi, Claudio/B-5654-2015; Leonidov, Andrey/P-3197-2014; Markina, Anastasia/E-3390-2012; Dogangun, Oktay/L-9252-2013; Marlow, Daniel/C-9132-2014; Oguri, Vitor/B-5403-2013; Janssen, Xavier/E-1915-2013; Bartalini, Paolo/E-2512-2014; Santoro, Alberto/E-7932-2014; Codispoti, Giuseppe/F-6574-2014; Max, Mad/E-5238-2010; Gribushin, Andrei/J-4225-2012; Cerrada, Marcos/J-6934-2014; Azzi, Patrizia/H-5404-2012; Sguazzoni, Giacomo/J-4620-2015; Ligabue, Franco/F-3432-2014; Fassi, Farida/F-3571-2016; Hernandez Calama, Jose Maria/H-9127-2015; Menasce, Dario Livio/A-2168-2016; Bargassa, Pedrame/O-2417-2016; Vilela Pereira, Antonio/L-4142-2016; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Goh, Junghwan/Q-3720-2016; 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Raidal, Martti/F-4436-2012; Tomei, Thiago/E-7091-2012; Zalewski, Piotr/H-7335-2013; Tinti, Gemma/I-5886-2013; Ivanov, Andrew/A-7982-2013; Hill, Christopher/B-5371-2012; Liu, Sheng/K-2815-2013; Venturi, Andrea/J-1877-2012; Wimpenny, Stephen/K-8848-2013; Alves, Gilvan/C-4007-2013; Tinoco Mendes, Andre David/D-4314-2011; Novaes, Sergio/D-3532-2012; Dudko, Lev/D-7127-2012; Mercadante, Pedro/K-1918-2012; Lokhtin, Igor/D-7004-2012; Della Ricca, Giuseppe/B-6826-2013; Kadastik, Mario/B-7559-2008; Mundim, Luiz/A-1291-2012; De La Cruz Burelo, Eduard/B-9802-2013; Petrushanko, Sergey/D-6880-2012; Santaolalla, Javier/C-3094-2013 OI Gonzi, Sandro/0000-0003-4754-645X; Heath, Helen/0000-0001-6576-9740; Scodellaro, Luca/0000-0002-4974-8330; Calvo Alamillo, Enrique/0000-0002-1100-2963; Paulini, Manfred/0000-0002-6714-5787; Vogel, Helmut/0000-0002-6109-3023; Marinho, Franciole/0000-0002-7327-0349; Ferguson, Thomas/0000-0001-5822-3731; Benussi, Luigi/0000-0002-2363-8889; Grandi, Claudio/0000-0001-5998-3070; Dogangun, Oktay/0000-0002-1255-2211; Codispoti, Giuseppe/0000-0003-0217-7021; Max, Mad/0000-0001-6966-6829; Cerrada, Marcos/0000-0003-0112-1691; Azzi, Patrizia/0000-0002-3129-828X; Sguazzoni, Giacomo/0000-0002-0791-3350; Casarsa, Massimo/0000-0002-1353-8964; Ligabue, Franco/0000-0002-1549-7107; Tricomi, Alessia Rita/0000-0002-5071-5501; Fassi, Farida/0000-0002-6423-7213; Heredia De La Cruz, Ivan/0000-0002-8133-6467; Ghezzi, Alessio/0000-0002-8184-7953; bianco, stefano/0000-0002-8300-4124; Covarelli, Roberto/0000-0003-1216-5235; Ciulli, Vitaliano/0000-0003-1947-3396; Fiorendi, Sara/0000-0003-3273-9419; Martelli, Arabella/0000-0003-3530-2255; Benaglia, Andrea Davide/0000-0003-1124-8450; Demaria, Natale/0000-0003-0743-9465; Hernandez Calama, Jose Maria/0000-0001-6436-7547; Bean, Alice/0000-0001-5967-8674; Longo, Egidio/0000-0001-6238-6787; Boccali, Tommaso/0000-0002-9930-9299; Menasce, Dario Livio/0000-0002-9918-1686; Bargassa, Pedrame/0000-0001-8612-3332; Attia Mahmoud, Mohammed/0000-0001-8692-5458; Bilki, Burak/0000-0001-9515-3306; Safdi, Benjamin R./0000-0001-9531-1319; Vilela Pereira, Antonio/0000-0003-3177-4626; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Gerbaudo, Davide/0000-0002-4463-0878; Vieira de Castro Ferreira da Silva, Pedro Manuel/0000-0002-5725-041X; Levchenko, Petr/0000-0003-4913-0538; Baarmand, Marc/0000-0002-9792-8619; Di Matteo, Leonardo/0000-0001-6698-1735; Diemoz, Marcella/0000-0002-3810-8530; TUVE', Cristina/0000-0003-0739-3153; KIM, Tae Jeong/0000-0001-8336-2434; Arce, Pedro/0000-0003-3009-0484; Flix, Josep/0000-0003-2688-8047; Paganoni, Marco/0000-0003-2461-275X; Gulmez, Erhan/0000-0002-6353-518X; Seixas, Joao/0000-0002-7531-0842; Sznajder, Andre/0000-0001-6998-1108; Lazzizzera, Ignazio/0000-0001-5092-7531; Sen, Sercan/0000-0001-7325-1087; D'Alessandro, Raffaello/0000-0001-7997-0306; Belyaev, Alexander/0000-0002-1733-4408; Stahl, Achim/0000-0002-8369-7506; Trocsanyi, Zoltan/0000-0002-2129-1279; Konecki, Marcin/0000-0001-9482-4841; Bedoya, Cristina/0000-0001-8057-9152; My, Salvatore/0000-0002-9938-2680; Matorras, Francisco/0000-0003-4295-5668; Ragazzi, Stefano/0000-0001-8219-2074; Wulz, Claudia-Elisabeth/0000-0001-9226-5812; Rolandi, Luigi (Gigi)/0000-0002-0635-274X; Montanari, Alessandro/0000-0003-2748-6373; Tomei, Thiago/0000-0002-1809-5226; Ivanov, Andrew/0000-0002-9270-5643; Hill, Christopher/0000-0003-0059-0779; Wimpenny, Stephen/0000-0003-0505-4908; Tinoco Mendes, Andre David/0000-0001-5854-7699; Novaes, Sergio/0000-0003-0471-8549; Dudko, Lev/0000-0002-4462-3192; Della Ricca, Giuseppe/0000-0003-2831-6982; Mundim, Luiz/0000-0001-9964-7805; De La Cruz Burelo, Eduard/0000-0002-7469-6974; FU Austrian Federal Ministry of Science and Research; Belgian Fonds de la Recherche Scientifique; Fonds voor Wetenschappelijk Onderzoek; CNPq; CAPES; FAPERJ; FAPESP; Bulgarian Ministry of Education and Science; CERN; Chinese Academy of Sciences; Ministry of Science and Technology; National Natural Science Foundation of China; Colombian Funding Agency (COLCIENCIAS); Croatian Ministry of Science, Education and Sport; Research Promotion Foundation, Cyprus; Ministry of Education and Research [SF0690030s09]; European Regional Development Fund, Estonia; Academy of Finland; Finnish Ministry of Education and Culture; Helsinki Institute of Physics; Institut National de Physique Nucleaire et de Physique des Particules/CNRS; Commissariat a l'Energie Atomique et aux Energies Alternatives/CEA, France; Bundesministerium fur Bildung und Forschung, Germany; Deutsche Forschungsgemeinschaft, Germany; Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; General Secretariat for Research and Technology, Greece; National Scientific Research Foundation; National Office for Research and Technology, Hungary; Department of Atomic Energy; Department of Science and Technology, India; Institute for Studies in Theoretical Physics and Mathematics, Iran; Science Foundation, Ireland; Istituto Nazionale di Fisica Nucleare, Italy; Korean Ministry of Education, Science and Technology; World Class University program of NRF, Korea; Lithuanian Academy of Sciences; CINVESTAV; CONACYT; SEP; UASLP-FAI; Ministry of Science and Innovation, New Zealand; Pakistan Atomic Energy Commission; Ministry of Science and Higher Education; National Science Centre, Poland; Fundacao para a Ciencia e a Tecnologia, Portugal;; JINR, Armenia; JINR, Belarus; JINR, Georgia; JINR, Ukraine; JINR, Uzbekistan; Ministry of Education and Science of the Russian Federation; Federal Agency of Atomic Energy of the Russian Federation; Russian Academy of Sciences; Russian Foundation for Basic Research; Ministry of Science and Technological Development of Serbia; Secretaria de Estado de Investigacion, Desarrollo e Innovacion, Spain; Programa Consolider-Ingenio, Spain; ETH Board; ETH Zurich; PSI; SNF; UniZH; Canton Zurich; SER; National Science Council, Taipei; Thailand Center of Excellence in Physics; Institute for the Promotion of Teaching Science and Technology; National Electronics and Computer Technology Center; Scientific and Technical Research Council of Turkey; Turkish Atomic Energy Authority; Science and Technology Facilities Council, UK; US Department of Energy; US National Science Foundation; Marie-Curie programme; European Research Council (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Austrian Science Fund (FWF); Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of Czech Republic; Council of Science and Industrial Research, India; Compagnia di San Paolo (Torino); HOMING PLUS programme of Foundation for Polish Science; European Union, Regional Development Fund FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC machine. We thank the technical and administrative staff at CERN and other CMS institutes. This work was supported by the Austrian Federal Ministry of Science and Research; the Belgian Fonds de la Recherche Scientifique, and Fonds voor Wetenschappelijk Onderzoek; the Brazilian Funding Agencies (CNPq, CAPES, FAPERJ, and FAPESP); the Bulgarian Ministry of Education and Science; CERN; the Chinese Academy of Sciences, Ministry of Science and Technology, and National Natural Science Foundation of China; the Colombian Funding Agency (COLCIENCIAS); the Croatian Ministry of Science, Education and Sport; the Research Promotion Foundation, Cyprus; the Ministry of Education and Research, Recurrent financing contract SF0690030s09 and European Regional Development Fund, Estonia; the Academy of Finland, Finnish Ministry of Education and Culture, and Helsinki Institute of Physics; the Institut National de Physique Nucleaire et de Physique des Particules/CNRS, and Commissariat a l'Energie Atomique et aux Energies Alternatives/CEA, France; the Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft, and Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; the General Secretariat for Research and Technology, Greece; the National Scientific Research Foundation, and National Office for Research and Technology, Hungary; the Department of Atomic Energy and the Department of Science and Technology, India; the Institute for Studies in Theoretical Physics and Mathematics, Iran; the Science Foundation, Ireland; the Istituto Nazionale di Fisica Nucleare, Italy; the Korean Ministry of Education, Science and Technology and the World Class University program of NRF, Korea; the Lithuanian Academy of Sciences; the Mexican Funding Agencies (CINVESTAV, CONACYT, SEP, and UASLP-FAI); the Ministry of Science and Innovation, New Zealand; the Pakistan Atomic Energy Commission; the Ministry of Science and Higher Education and the National Science Centre, Poland; the Fundacao para a Ciencia e a Tecnologia, Portugal; JINR (Armenia, Belarus, Georgia, Ukraine, Uzbekistan); the Ministry of Education and Science of the Russian Federation, the Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences, and the Russian Foundation for Basic Research; the Ministry of Science and Technological Development of Serbia; the Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio 2010, Spain; the Swiss Funding Agencies (ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER); the National Science Council, Taipei; the Thailand Center of Excellence in Physics, the Institute for the Promotion of Teaching Science and Technology and National Electronics and Computer Technology Center; the Scientific and Technical Research Council of Turkey, and Turkish Atomic Energy Authority; the Science and Technology Facilities Council, UK; the US Department of Energy, and the US National Science Foundation.; Individuals have received support from the Marie-Curie programme and the European Research Council (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Austrian Science Fund (FWF); the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of Czech Republic; the Council of Science and Industrial Research, India; the Compagnia di San Paolo (Torino); and the HOMING PLUS programme of Foundation for Polish Science, cofinanced from European Union, Regional Development Fund. NR 71 TC 8 Z9 8 U1 3 U2 77 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD NOV PY 2012 IS 11 AR 147 DI 10.1007/JHEP11(2012)147 PG 47 WC Physics, Particles & Fields SC Physics GA 056JL UT WOS:000312484500016 ER PT J AU Franco, S AF Franco, Sebastian TI Bipartite field theories: from D-brane probes to scattering amplitudes SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Supersymmetric gauge theory; Duality in Gauge Field Theories ID GAUGE-THEORIES; DUALITY AB We introduce and initiate the investigation of a general class of 4d, N = 1 quiver gauge theories whose Lagrangian is defined by a bipartite graph on a Riemann surface, with or without boundaries. We refer to such class of theories as Bipartite Field Theories (BFTs). BFTs underlie a wide spectrum of interesting physical systems, including: D3-branes probing tonic Calabi-Yau 3-folds, their mirror configurations of D6-branes, cluster integrable systems in (0+1) dimensions and leading singularities in scattering amplitudes for N = 4 SYM. While our discussion is fully general, we focus on models that are relevant for scattering amplitudes. We investigate the BFT perspective on graph modifications, the emergence of Calabi-Yau manifolds (which arise as the master and moduli spaces of BFT's), the translation between square moves in the graph and Seiberg duality and the identification of dual theories by means of the underlying Calabi-Yaus, the phenomenon of loop reduction and the interpretation of the boundary operator for cells in the positive Grassmannian as higgsing in the BFT. We develop a technique based on generalized Kasteleyn matrices that permits an efficient determination of the Calabi-Yau geometries associated to arbitrary graphs. Our techniques allow us to go beyond the planar limit by both increasing the number of boundaries of the graphs and the genus of the underlying Riemann surface. Our investigation suggests a central role for Calabi-Yau manifolds in the context of leading singularities, whose full scope is yet to be uncovered. C1 [Franco, Sebastian] Stanford Linear Accelerator Ctr, Natl Accelerator Lab, Theory Grp, Menlo Pk, CA 94309 USA. [Franco, Sebastian] Univ Durham, Dept Phys, Inst Particle Phys Phenomenol, Durham DH1 3LE, England. RP Franco, S (reprint author), Stanford Linear Accelerator Ctr, Natl Accelerator Lab, Theory Grp, Menlo Pk, CA 94309 USA. EM sfranco@slac.stanford.edu FU US DOE [DE-AC02-76SF00515]; U.K. Science and Technology Facilities Council (STFC) FX We would like to thank J. Bourjaily, J. Kaplan and L. Williams for useful correspondence and explanations, and D. Galloni and R.-K. Seong for interesting discussions and collaboration on a related project. We are particularly thankful to N. Arkani-Hamed for very useful correspondence. Finally, we thank D. Xie and M. Yamazaki for informing us about their upcoming work [57], and sharing a draft of it prior to publication. This work was supported by the US DOE under contract number DE-AC02-76SF00515 and by the U.K. Science and Technology Facilities Council (STFC). NR 55 TC 23 Z9 23 U1 1 U2 2 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD NOV PY 2012 IS 11 AR 141 DI 10.1007/JHEP11(2012)141 PG 49 WC Physics, Particles & Fields SC Physics GA 056JL UT WOS:000312484500010 ER PT J AU Choi, YB Hinoki, T Ozawa, K Katoh, Y Matsugi, K Kelimu, T AF Choi, Y. B. Hinoki, T. Ozawa, K. Katoh, Y. Matsugi, K. Kelimu, T. TI Strength Anisotropy of NITE-SiC/SiC Composite by Various Failure Modes SO MATERIALS TRANSACTIONS LA English DT Article DE SiC/SiC composite; trans-thickness tensile strength; inter-laminar shear strength; tensile strength; anisotropy AB SiC/SiC composite is a candidate material for demonstration fusion power reactor (DEMO). To identify the inherent anisotropy of composites, it requires predicting axial/off-axial mechanical properties by various failure modes. This study evaluated failure behavior of SiC/SiC composites by various mode tests such as tensile, Inter-laminar shear and Trans-thickness tensile modes. To provide strength anisotropy maps and discussed a method to predict this trend analytically. The identification of various fabric orientations from strength anisotropy maps clearly indicate that the composites failed by the mixed modes. The strength anisotropy can be described satisfactorily. [doi:10.2320/matertrans.M2012182] C1 [Choi, Y. B.; Matsugi, K.] Hiroshima Univ, Dept Mech Syst Engn, Higasi Hiroshima 7398527, Japan. [Hinoki, T.] Kyoto Univ, Inst Adv Energy, Kyoto 6110011, Japan. [Ozawa, K.; Katoh, Y.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Kelimu, T.] Gyeongsang Natl Univ, Dept Mech & Precis Engn, Tongyeong, South Korea. RP Choi, YB (reprint author), Hiroshima Univ, Dept Mech Syst Engn, Higasi Hiroshima 7398527, Japan. EM ybchoi@hiroshima-u.ac.jp RI Choi, yongbum/D-7189-2011; Matsugi, Kazuhiro/D-8748-2012 NR 8 TC 2 Z9 2 U1 0 U2 9 PU JAPAN INST METALS PI SENDAI PA 1-14-32, ICHIBANCHO, AOBA-KU, SENDAI, 980-8544, JAPAN SN 1345-9678 EI 1347-5320 J9 MATER TRANS JI Mater. Trans. PD NOV PY 2012 VL 53 IS 11 BP 2060 EP 2063 DI 10.2320/matertrans.M2012182 PG 4 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA 060FB UT WOS:000312760800041 ER PT J AU Deng, L Gregory, A Yilmaz, S Poulos, BT Hugenholtz, P Sullivan, MB AF Deng, Li Gregory, Ann Yilmaz, Suzan Poulos, Bonnie T. Hugenholtz, Philip Sullivan, Matthew B. TI Contrasting Life Strategies of Viruses that Infect Photo- and Heterotrophic Bacteria, as Revealed by Viral Tagging SO MBIO LA English DT Article ID ESCHERICHIA-COLI O157-H7; MARINE VIRUSES; PHOTOSYNTHESIS GENES; CYANOBACTERIUM PROCHLOROCOCCUS; MICROBIAL COMMUNITIES; NORTH-SEA; DIVERSITY; PHAGE; GENOME; OCEAN AB Ocean viruses are ubiquitous and abundant and play important roles in global biogeochemical cycles by means of their mortality, horizontal gene transfer, and manipulation of host metabolism. However, the obstacles involved in linking viruses to their hosts in a high-throughput manner bottlenecks our ability to understand virus-host interactions in complex communities. We have developed a method called viral tagging (VT), which combines mixtures of host cells and fluorescent viruses with flow cytometry. We investigated multiple viruses which infect each of two model marine bacteria that represent the slow-growing, photoautotrophic genus Synechococcus (Cyanobacteria) and the fast-growing, heterotrophic genus Pseudoalteromonas (Gammaproteobacteria). Overall, viral tagging results for viral infection were consistent with plaque and liquid infection assays for cyanobacterial myo-, podo- and siphoviruses and some (myo- and podoviruses) but not all (four siphoviruses) heterotrophic bacterial viruses. Virus-tagged Pseudoalteromonas organisms were proportional to the added viruses under varied infection conditions (virus-bacterium ratios), while no more than 50% of the Synechococcus organisms were virus tagged even at viral abundances that exceeded (5 to 10x) that of their hosts. Further, we found that host growth phase minimally impacts the fraction of virus-tagged Synechococcus organisms while greatly affecting phage adsorption to Pseudoalteromonas. Together these findings suggest that at least two contrasting viral life strategies exist in the oceans and that they likely reflect adaptation to their host microbes. Looking forward to the point at which the virus-tagging signature is well understood (e. g., for Synechococcus), application to natural communities should begin to provide population genomic data at the proper scale for predictively modeling two of the most abundant biological entities on Earth. IMPORTANCE Viral study suffers from an inability to link viruses to hosts en masse, and yet delineating "who infects whom" is fundamental to viral ecology and predictive modeling. This article describes viral tagging-a high-throughput method to investigate virus-host interactions by combining the fluorescent labeling of viruses for "tagging" host cells that can be analyzed and sorted using flow cytometry. Two cultivated hosts (the cyanobacterium Synechococcus and the gammaproteobacterium Pseudoalteromonas) and their viruses (podo-, myo-, and siphoviruses) were investigated to validate the method. These lab-based experiments indicate that for most virus-host pairings, VT (viral tagging) adsorption is equivalent to traditional infection by liquid and plaque assays, with the exceptions being confined to promiscuous adsorption by Pseudoalteromonas siphoviruses. These experiments also reveal variability in life strategies across these oceanic virus-host systems with respect to infection conditions and host growth status, which highlights the need for further model system characterization to break open this virus-host interaction "black box." C1 [Deng, Li; Gregory, Ann; Poulos, Bonnie T.; Sullivan, Matthew B.] Univ Arizona, Ecol & Evolutionary Biol Dept, Tucson, AZ USA. [Yilmaz, Suzan; Hugenholtz, Philip] US DOE, Microbial Ecol Program, Joint Genome Inst, Walnut Creek, CA USA. [Hugenholtz, Philip] Univ Queensland, Australian Ctr Ecogen, Sch Chem & Mol Biosci, St Lucia, Qld, Australia. [Hugenholtz, Philip] Univ Queensland, Inst Mol Biosci, St Lucia, Qld, Australia. RP Hugenholtz, P (reprint author), US DOE, Microbial Ecol Program, Joint Genome Inst, Walnut Creek, CA USA. EM hugenholtz@uq.edu.au; mbsulli@email.arizona.edu RI Hugenholtz, Philip/G-9608-2011; Sullivan, Matthew/H-3256-2011 OI Sullivan, Matthew/0000-0003-4040-9831 FU Biosphere 2; BIO5; NSF [OCE0940390]; Gordon and Betty Moore Foundation; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Biosphere 2, BIO5, NSF OCE0940390, and a Gordon and Betty Moore Foundation grant to M. B. S. The work conducted by the U.S. Department of Energy Joint Genome Institute was supported by the Office of Science of the U.S. Department of Energy under contract no. DE-AC02-05CH11231. NR 77 TC 32 Z9 34 U1 6 U2 66 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 2150-7511 J9 MBIO JI mBio PD NOV-DEC PY 2012 VL 3 IS 6 AR e00373-12 DI 10.1128/mBio.00373-12 PG 8 WC Microbiology SC Microbiology GA 064UK UT WOS:000313100700010 ER PT J AU Payne, SH Bonissone, S Wu, S Brown, RN Ivankov, DN Frishman, D Pasa-Tolic, L Smith, RD Pevzner, PA AF Payne, Samuel H. Bonissone, Stefano Wu, Si Brown, Roslyn N. Ivankov, Dmitry N. Frishman, Dmitrij Pasa-Tolic, Ljiljana Smith, Richard D. Pevzner, Pavel A. TI Unexpected Diversity of Signal Peptides in Prokaryotes SO MBIO LA English DT Article ID TANDEM MASS-SPECTRA; CLEAVAGE SITES; IDENTIFICATION; SEQUENCE; PROTEIN AB Signal peptides are a cornerstone mechanism for cellular protein localization, yet until now experimental determination of signal peptides has come from only a narrow taxonomic sampling. As a result, the dominant view is that Sec-cleaved signal peptides in prokaryotes are defined by a canonical AxA motif. Although other residues are permitted in the motif, alanine is by far the most common. Here we broadly examine proteomics data to reveal the signal peptide sequences for 32 bacterial and archaeal organisms from nine phyla and demonstrate that this alanine preference is not universal. Discoveries include fundamentally distinct signal peptide motifs from Alphaproteobacteria, Spirochaetes, Thermotogae and Euryarchaeota. In these novel motifs, alanine is no longer the dominant residue but has been replaced in a different way for each taxon. Surprisingly, divergent motifs correlate with a proteome-wide reduction in alanine. Computational analyses of similar to 1,500 genomes reveal numerous major evolutionary clades which have replaced the canonical signal peptide sequence with novel motifs. IMPORTANCE This article replaces a widely held general model with a more detailed model describing phylogenetically correlated variation in motifs for Sec secretion. C1 [Payne, Samuel H.; Brown, Roslyn N.; Smith, Richard D.] Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99352 USA. [Bonissone, Stefano; Pevzner, Pavel A.] Univ Calif San Diego, Bioinformat Program, La Jolla, CA 92093 USA. [Wu, Si; Pasa-Tolic, Ljiljana] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Ivankov, Dmitry N.; Frishman, Dmitrij] Tech Univ Munich, Dept Genome Oriented Bioinformat, D-80290 Munich, Germany. [Frishman, Dmitrij] German Res Ctr Environm Hlth, Helmholtz Ctr Munich, Inst Bioinformat & Syst Biol, Neuherberg, Germany. [Pevzner, Pavel A.] Univ Calif San Diego, Dept Comp Sci & Engn, La Jolla, CA 92093 USA. RP Payne, SH (reprint author), Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99352 USA. EM samuel.payne@pnnl.gov RI Smith, Richard/J-3664-2012; OI Smith, Richard/0000-0002-2381-2349; Payne, Samuel/0000-0002-8351-1994 FU NSF [EF-0949047]; DOE by Battelle [DEAC05-76RLO 1830] FX This work was supported by an NSF award to S. H. P. (EF-0949047). Data from the Pacific Northwest National Laboratory were obtained in the Environmental Molecular Sciences Laboratory, a U.S. Department of Energy/Biological and Environmental Research national scientific user facility. Pacific Northwest National Laboratory is operated for the DOE by Battelle under contract DEAC05-76RLO 1830. NR 19 TC 6 Z9 6 U1 0 U2 11 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 2150-7511 J9 MBIO JI mBio PD NOV-DEC PY 2012 VL 3 IS 6 AR e00339-12 DI 10.1128/mBio.00339-12 PG 6 WC Microbiology SC Microbiology GA 064UK UT WOS:000313100700007 ER PT J AU Wattam, AR Inzana, TJ Williams, KP Mane, SP Shukla, M Almeida, NF Dickerman, AW Mason, S Moriyon, I O'Callaghan, D Whatmore, AM Sobral, BW Tiller, RV Hoffmaster, AR Frace, MA De Castro, C Molinaro, A Boyle, SM De, BK Setubal, JC AF Wattam, Alice R. Inzana, Thomas J. Williams, Kelly P. Mane, Shrinivasrao P. Shukla, Maulik Almeida, Nalvo F. Dickerman, Allan W. Mason, Steven Moriyon, Ignacio O'Callaghan, David Whatmore, Adrian M. Sobral, Bruno W. Tiller, Rebekah V. Hoffmaster, Alex R. Frace, Michael A. De Castro, Cristina Molinaro, Antonio Boyle, Stephen M. De, Barun K. Setubal, Joao C. TI Comparative Genomics of Early-Diverging Brucella Strains Reveals a Novel Lipopolysaccharide Biosynthesis Pathway (vol 3, e00246, 2012) SO MBIO LA English DT Correction C1 [Wattam, Alice R.; Mane, Shrinivasrao P.; Shukla, Maulik; Dickerman, Allan W.; Mason, Steven; Sobral, Bruno W.; Setubal, Joao C.] Virginia Tech, Virginia Bioinformat Inst, Blacksburg, VA USA. [Inzana, Thomas J.; Boyle, Stephen M.] Virginia Tech, Ctr Mol Med & Infect Dis, Virginia Maryland Reg Coll Vet Med, Blacksburg, VA 24061 USA. [Williams, Kelly P.] Sandia Natl Labs, Livermore, CA USA. [Almeida, Nalvo F.] Univ Fed Mato Grosso do Sul, Fac Comp, Campo Grande, MS, Brazil. [Moriyon, Ignacio] Univ Navarra, Inst Salud Trop, Fac Med, E-31080 Pamplona, Spain. [Moriyon, Ignacio] Univ Navarra, Dept Microbiol & Parasitol, Fac Med, E-31080 Pamplona, Spain. [O'Callaghan, David] INSERM, U1047, UFR Med, Nimes, France. [O'Callaghan, David] Univ Montpellier I, UFR Med, Nimes, France. [Whatmore, Adrian M.] Anim Hlth & Vet Labs Agcy, Dept Bacteriol, Addlestone, Surrey, England. [Tiller, Rebekah V.; Hoffmaster, Alex R.; Frace, Michael A.; De, Barun K.] Ctr Dis Control & Prevent, Atlanta, GA USA. [De Castro, Cristina; Molinaro, Antonio] Univ Naples Federico II, Dept Chem Sci, Naples, Italy. [Setubal, Joao C.] Univ Sao Paulo, Dept Biochem, Inst Chem, Sao Paulo, Brazil. RP Inzana, TJ (reprint author), Virginia Tech, Ctr Mol Med & Infect Dis, Virginia Maryland Reg Coll Vet Med, Blacksburg, VA 24061 USA. EM tinzana@vt.edu RI Setubal, Joao/C-7305-2012; Moriyon, Ignacio/N-4764-2016 OI Setubal, Joao/0000-0001-9174-2816; Moriyon, Ignacio/0000-0002-4288-0195 NR 1 TC 0 Z9 0 U1 0 U2 4 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 2150-7511 J9 MBIO JI mBio PD NOV-DEC PY 2012 VL 3 IS 6 AR e00388-12 DI 10.1128/mBio.00388 PG 1 WC Microbiology SC Microbiology GA 064UK UT WOS:000313100700014 ER PT J AU Panessa-Warren, BJ Warren, JB Kisslinger, K Crosson, K Maye, MM AF Panessa-Warren, Barbara J. Warren, John B. Kisslinger, Kim Crosson, Kenya Maye, Mathew M. TI Human Airway Epithelial Cell Responses to Single Walled Carbon Nanotube Exposure: Nanorope-Residual Body Formation SO NANOSCIENCE AND NANOTECHNOLOGY LETTERS LA English DT Article DE Single Walled Carbon Nanotubes; Human Lung Epithelium; Nanorope-Residual Body ID NANOPARTICULATE MATERIALS; ELECTRON-MICROSCOPY; OXIDATIVE STRESS; RAT LUNG; CYTOTOXICITY; NICKEL; APOPTOSIS; TOXICITY AB This investigation examines the 'first contact responses' of in vitro human epithelial airway cells exposed to unrefined single walled carbon nanotubes (SWCNTs) [containing metal catalyst, carbon black, amorphous carbon, graphitic shells, and SWCNTs], and refined acid/peroxide cleaned and cut SWCNTs at low and high dose exposures (0.16 ug/L and 1.60 ug/L) for 2, 3 and 3.5 hours. FTIR, X-ray compositional analysis, morphological TEM analysis and UV-Vis were used to physicochemically characterize the SWCNTs in this study. Following SWCNT exposure to human lung NCl-H292 epithelial monolayers, the airway cells were prepared for light microscopy vital staining, or fixed in glutaraldehyde for SEM/TEM imaging to determine SWCNT binding, uptake, intracellular processing and organellar/SWCNT fate within the exposure period. At 2 hr exposures to both unrefined Carbolex, and refined SWCNTs (at both high and low doses), there were no increases in lung cell necrosis compared to controls. However high dose, 3 hr exposures to unrefined Carbolex material produced severe cell damage (apical and basal plasma membrane holes, decreased mitochondria, numerous intracellular vesicles containing nanomaterial and membrane fragments) and increased cell necrosis. The refined SWCNTs exposed for 3 hr at low dose produced no increase in cell death, although high dose exposure produced significant cell death. By TEM, Acid/peroxide cleaned SWCNT 3 hr exposures at high and low doses, revealed SWCNTs attachment to cell surface mucin, and SWCNT uptake into the cells during membrane recycling. Membranes and SWCNTs were seen within cytoplasmic lamellar body-type vesicles, where vesicular contents were bio-degraded, eventually forming long SWCNT-nanoropes, which were subsequently released into the cytoplasm as clusters of attached nanoropes, as the vesicle membranes fragmented. These Nanorope-Residual Bodies did not cause damage to the surrounding organelles or cytoplasm, and seemed very stabile in the cell cytoplasm. To our knowledge this is the first time that human lung cells have been shown to very rapidly bind, incorporate, bio-degrade and re-assemble SWCNTs into nanoropes intracellularly, to form stabile Nanorope Residual bodies. C1 [Panessa-Warren, Barbara J.] Brookhaven Natl Lab, Dept Sustainable Energy Technol, Upton, NY 11973 USA. [Warren, John B.] Brookhaven Natl Lab, Instrumentat Div, Upton, NY 11973 USA. [Kisslinger, Kim] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Crosson, Kenya] Univ Dayton, Dept Environm Engn & Engn Mech, Dayton, OH 45469 USA. [Maye, Mathew M.] Syracuse Univ, Dept Chem, Syracuse, NY 13244 USA. RP Panessa-Warren, BJ (reprint author), Brookhaven Natl Lab, Dept Sustainable Energy Technol, POB 5000, Upton, NY 11973 USA. RI Kisslinger, Kim/F-4485-2014 FU U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886]; DOE Laboratory Directed Research Development [2850] FX This Research was carried out (in part) at the Center for Functional Nanomaterials, the Instrumentation Division and at the Department of Sustainable Energy Technologies, at Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886.; The authors would like to acknowledge and thank Dr. Veljko Radeka for the use of laboratory space and equipment in the Instrumentation Division at Brookhaven National Laboratory where much of the work for this investigation was done; Dr. Oleg Gang and Dr. Mathew Maye who were instrumental in doing the FTIR, UV-Vis and DLS measurements at the Center for Functional Nanomaterials (CFN) at Brookhaven; and at the CFN Mr. Kim Kiss linger, Dr. Lihua Zhang and Dr. Eli Sutter for their microscopy assistance, and discussions about the data collected using the JEOL 1400 and JEOL JSM 2100F HRTEM, X-ray elemental analysis system and TEM electron diffraction. and Dr. J. Patrick Looney and Dr. Robert Lofaro (Department of Sustainable Energy Technologies) and Dr. William Horak (Department of Nuclear Energy Sciences) in the Global and Regional Solutions Directorate at Brookhaven National Laboratory, who also made this work possible. The original study was funded by a DOE Laboratory Directed Research Development Grant (number 2850). NR 38 TC 4 Z9 4 U1 0 U2 15 PU AMER SCIENTIFIC PUBLISHERS PI VALENCIA PA 26650 THE OLD RD, STE 208, VALENCIA, CA 91381-0751 USA SN 1941-4900 J9 NANOSCI NANOTECH LET JI Nanosci. Nanotechnol. Lett. PD NOV PY 2012 VL 4 IS 11 BP 1110 EP 1121 DI 10.1166/nnl.2012.1469 PG 12 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA 063AA UT WOS:000312965600015 ER PT J AU Luk, KB AF Luk, Kam-Biu TI Towards a theta(13) measurement SO PRAMANA-JOURNAL OF PHYSICS LA English DT Article DE Reactor; neutrino; oscillation; mixing AB Reactor-based antineutrino experiments hold the promise of providing an unambiguous determination of the neutrino mixing angle theta (13). At present, Daya Bay, Double Chooz and RENO are such experiments being set up for this purpose. In this paper, the status and prospects of these three initiatives are presented. C1 [Luk, Kam-Biu] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Luk, Kam-Biu] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. RP Luk, KB (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM k_luk@lbl.gov FU Office of Science, Office of High Energy Physics, of the US Department of Energy [DE-AC02-05CH11231, DE-FG02-94ER40840] FX The author would like to thank Herve de Kerret, Soo-Boo Kim, Takashi Kobayashi and the Daya Bay Collaborations for providing updated information to prepare the presentation. In addition, the author would like to thank Office of Science, Office of High Energy Physics, of the US Department of Energy under Contract No. DE-AC02-05CH11231 and Contract No. DE-FG02-94ER40840 for funding support. NR 10 TC 0 Z9 0 U1 0 U2 0 PU INDIAN ACAD SCIENCES PI BANGALORE PA C V RAMAN AVENUE, SADASHIVANAGAR, P B #8005, BANGALORE 560 080, INDIA SN 0304-4289 EI 0973-7111 J9 PRAMANA-J PHYS JI Pramana-J. Phys. PD NOV PY 2012 VL 79 IS 5 BP 963 EP 977 DI 10.1007/s12043-012-0412-4 PG 15 WC Physics, Multidisciplinary SC Physics GA 055RW UT WOS:000312435600003 ER PT J AU Mahajan, S Kumar, A Raja, R AF Mahajan, Sonam Kumar, Ashok Raja, Rajendran TI Main injector particle production experiment at Fermilab SO PRAMANA-JOURNAL OF PHYSICS LA English DT Article DE Main injector particle production; neutrinos; neutrons; NuMI; KNO AB The main injector particle production (MIPP) experiment at Fermilab uses particle beams of charged pions, kaons, proton and antiproton with beam momenta of 5-90 GeV/c to measure particle production cross-sections of various nuclei including liquid hydrogen, MINOS target and thin targets of beryllium, carbon, bismuth and uranium. The physics motivation to perform such cross-section measurements is described here. Recent results on the analysis of NuMI target and forward neutron cross-sections are presented here. Preliminary cross-section measurements for 58 GeV/c proton on liquid hydrogen target are also presented. A new method is described to correct for low multiplicity inefficiencies in the trigger using KNO scaling. C1 [Mahajan, Sonam; Kumar, Ashok] Panjab Univ, Dept Phys, Chandigarh 160014, India. [Raja, Rajendran] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. RP Kumar, A (reprint author), Panjab Univ, Dept Phys, Chandigarh 160014, India. EM ashok@pu.ac.in FU Fermilab under India-Fermilab Neutrino Collaboration FX This work is supported by Fermilab under India-Fermilab Neutrino Collaboration. NR 4 TC 0 Z9 0 U1 0 U2 2 PU INDIAN ACAD SCIENCES PI BANGALORE PA C V RAMAN AVENUE, SADASHIVANAGAR, P B #8005, BANGALORE 560 080, INDIA SN 0304-4289 J9 PRAMANA-J PHYS JI Pramana-J. Phys. PD NOV PY 2012 VL 79 IS 5 BP 1243 EP 1246 DI 10.1007/s12043-012-0432-0 PG 4 WC Physics, Multidisciplinary SC Physics GA 055RW UT WOS:000312435600023 ER PT J AU Jeon, M Kim, Y Hwang, J Lee, J Seo, E AF Jeon, Myeongjae Kim, Youngjae Hwang, Jeaho Lee, Joonwon Seo, Euiseong TI Workload Characterization and Performance Implications of Large-Scale Blog Servers SO ACM TRANSACTIONS ON THE WEB LA English DT Article DE Design; Measurement; Performance; Social network services; workload characterization; measurement; modeling; filesystems AB With the ever-increasing popularity of Social Network Services (SNSs), an understanding of the characteristics of these services and their effects on the behavior of their host servers is critical. However, there has been a lack of research on the workload characterization of servers running SNS applications such as blog services. To fill this void, we empirically characterized real-world Web server logs collected from one of the largest South Korean blog hosting sites for 12 consecutive days. The logs consist of more than 96 million HTTP requests and 4.7TB of network traffic. Our analysis reveals the following: (i) The transfer size of nonmultimedia files and blog articles can be modeled using a truncated Pareto distribution and a log-normal distribution, respectively; (ii) user access for blog articles does not show temporal locality, but is strongly biased towards those posted with image or audio files. We additionally discuss the potential performance improvement through clustering of small files on a blog page into contiguous disk blocks, which benefits from the observed file access patterns. Trace-driven simulations show that, on average, the suggested approach achieves 60.6% better system throughput and reduces the processing time for file access by 30.8% compared to the best performance of the Ext4 filesystem. C1 [Lee, Joonwon; Seo, Euiseong] Sungkyunkwan Univ, Coll Informat & Commun Engn, Seoul, South Korea. [Jeon, Myeongjae] Rice Univ, Dept Comp Sci, Houston, TX 77251 USA. [Kim, Youngjae] Oak Ridge Natl Lab, Oak Ridge, TN USA. [Hwang, Jeaho] Korea Adv Inst Sci & Technol, Dept Comp Sci, Taejon, South Korea. RP Seo, E (reprint author), Sungkyunkwan Univ, Coll Informat & Commun Engn, Seoul, South Korea. EM euiseong@gmail.com FU MKE/KEIT [10041244]; Next-Generation Information Computing Development program through the NRF; MEST [2012-0006423]; Office of Science of the U.S. Department of Energy [DE-AC05-00OR22725] FX This work was partly supported by the IT R&D program of MKE/KEIT [10041244, Smart TV 2.0 Software Platform], the Next-Generation Information Computing Development program through the NRF funded by the MEST (2012-0006423), and partially through the Office of Science of the U.S. Department of Energy under Contract No. DE-AC05-00OR22725. NR 39 TC 2 Z9 2 U1 0 U2 11 PU ASSOC COMPUTING MACHINERY PI NEW YORK PA 2 PENN PLAZA, STE 701, NEW YORK, NY 10121-0701 USA SN 1559-1131 J9 ACM T WEB JI ACM Trans. Web PD NOV PY 2012 VL 6 IS 4 AR 16 DI 10.1145/2382616.2382619 PG 26 WC Computer Science, Information Systems; Computer Science, Software Engineering SC Computer Science GA 055KP UT WOS:000312415300003 ER PT J AU Varshney, D Sumant, AV Weiner, BR Morell, G AF Varshney, Deepak Sumant, Anirudha V. Weiner, Brad R. Morell, Gerardo TI Growth of carbon nanotubes on spontaneously detached free standing diamond films and their field emission properties SO DIAMOND AND RELATED MATERIALS LA English DT Article DE Carbon nanotubes; Diamond; Hot filament chemical vapor deposition; Field Emission ID CVD; ENHANCEMENT; NANODIAMOND; DEPOSITION; STABILITY; EMITTERS AB Carbon nanotubes (CNTs) have been fabricated on free-standing microcrystalline diamond (FSD) films by hot filament chemical vapor deposition using Ni as catalyst. Micro Raman spectroscopy has been used as a primary technique to characterize the hybrid material, while electron microscopy and electron energy loss spectroscopy served as complementary characterization techniques. The fabricated material shows the presence of multiwall carbon nanotubes of diameters in the range of 10-15 nm with a wall thickness of 5-6 nm protruding from the free-standing microcrystalline diamond films of crystallite sizes ranging from 0.5 to 2.0 mu m. The CNT-FSD films show good field emission properties with low turn-on field, large field enhancement factor, and an excellent current stability over a period of 10 days. Published by Elsevier B.V. C1 [Varshney, Deepak; Weiner, Brad R.; Morell, Gerardo] Univ Puerto Rico, Dept Phys, San Juan, PR 00936 USA. [Varshney, Deepak; Morell, Gerardo] Univ Puerto Rico, Inst Funct Nanomat, San Juan, PR 00931 USA. [Sumant, Anirudha V.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Weiner, Brad R.] Univ Puerto Rico, Dept Chem, San Juan, PR 00936 USA. RP Varshney, D (reprint author), Univ Puerto Rico, Dept Phys, POB 70377, San Juan, PR 00936 USA. EM deepvar20@gmail.com RI Morell, Gerardo/H-6300-2011 OI Morell, Gerardo/0000-0003-4787-2239 FU Institute for Functional Nanomaterials (NSF Grant) [1002410]; PR NASA EPSCoR (NASA) [NNX07AO30A, NNX08BA48A]; PR DOE EPSCoR (DOE Grant) [DEFG02-08ER46526]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This research was made possible by funds from the Institute for Functional Nanomaterials (NSF Grant # 1002410), PR NASA EPSCoR (NASA Cooperative Agreements # NNX07AO30A and NNX08BA48A), and PR DOE EPSCoR (DOE Grant # DEFG02-08ER46526). We would like to acknowledge the help of Mr. W. Perez with the Raman spectroscopy measurements and Mr. Frank Mendoza with the SEM measurements. Use of the Center for Nanoscale Materials was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 39 TC 9 Z9 9 U1 1 U2 36 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0925-9635 J9 DIAM RELAT MATER JI Diam. Relat. Mat. PD NOV PY 2012 VL 30 BP 42 EP 47 DI 10.1016/j.diamond.2012.09.009 PG 6 WC Materials Science, Multidisciplinary SC Materials Science GA 056TP UT WOS:000312514600007 ER PT J AU Colgan, J Pindzola, MS AF Colgan, J. Pindzola, M. S. TI Application of the time-dependent close-coupling approach to few-body atomic and molecular ionizing collisions SO EUROPEAN PHYSICAL JOURNAL D LA English DT Article ID ELECTRON-IMPACT IONIZATION; DIFFERENTIAL CROSS-SECTIONS; PHOTO-DOUBLE-IONIZATION; 2-PHOTON DOUBLE-IONIZATION; CORRELATED PHOTOIONIZATION PROCESSES; NEAR-THRESHOLD; R-MATRIX; DISSOCIATIVE IONIZATION; TRIPLE PHOTOIONIZATION; INTERMEDIATE ENERGIES AB We review the recent progress made in applying the time-dependent close-coupling approach to ionizing collisions of electrons, photons, and ions with small atoms and molecules. The last twenty years have seen a proliferation of non-perturbative approaches applied to fundamental atomic and molecular scattering processes. Such processes form the building blocks of describing the dynamics of plasmas over a wide range of temperatures and densities, and also provide insight into the long-range Coulomb interactions between charged particles. Studies of the few-body Coulomb problem presented in electron, photon, or ion-impact ionization of small atoms and molecules, by direct solution of the time-dependent Schrodinger equation, are particularly useful because the complicated three-body boundary conditions of more than one continuum particle in a Coulomb potential are not required. With the continuing growth and increasing availability of high-performance computing resources, such methods can now be applied to a wide variety of scattering processes. The recent progress made using such a time-dependent approach is described in this colloquium. In this paper, we focus on the recent results obtained for one-, two-, and three-electron systems, thus building on a previous review of the time-dependent close-coupling method [M. S. Pindzola et al., J. Phys. B 40, R39 (2007)], which also described the application to multi-electron targets. C1 [Colgan, J.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Pindzola, M. S.] Auburn Univ, Dept Phys, Auburn, AL 36849 USA. RP Colgan, J (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM jcolgan@lanl.gov OI Colgan, James/0000-0003-1045-3858 FU NNSA of the U.S. DOE [DE-AC5206NA25396]; U.S. DOE; U.S. NSF FX We are grateful for long-standing collaborations with many researchers in the atomic collision field over the years, and in particular wish to thank F. Robicheaux, D. C. Griffin, C. P. Ballance, S. D. Loch, D. Schultz, G.S.J. Armstrong, C.J. Fontes, J.C. Berengut, T. Topcu, M. Foster, T. Minami, N.R. Badnell, M. C. Witthoeft, D. R. Plante, D. M. Mitnik, J.A. Ludlow, U. Kleiman, T. G. Lee, and Sh.A. Abdel-Naby. The Los Alamos National Laboratory is operated by Los Alamos National Security, LLC for the NNSA of the U.S. DOE under Contract No. DE-AC5206NA25396. Much of the work described here was supported in part by grants from the U.S. DOE and from the U.S. NSF to Auburn University. Computational work was carried out at the NERSC in Oakland, California, the NICS in Knoxville, Tennessee, and at Los Alamos National Laboratory. NR 188 TC 22 Z9 22 U1 0 U2 14 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6060 J9 EUR PHYS J D JI Eur. Phys. J. D PD NOV PY 2012 VL 66 IS 11 AR 284 DI 10.1140/epjd/e2012-30517-2 PG 24 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA 055SY UT WOS:000312439000004 ER PT J AU Sagot, MF AF Sagot, Marie-France TI EIC Editorial SO IEEE-ACM TRANSACTIONS ON COMPUTATIONAL BIOLOGY AND BIOINFORMATICS LA English DT Editorial Material C1 GRAIL, Oak Ridge Natl Lab, Oak Ridge, TN USA. Univ Tecn Lisboa, IST, P-1100 Lisbon, Portugal. Univ Calif Riverside, Dept Comp Sci & Engn, Riverside, CA 92521 USA. Univ Kansas, Lawrence, KS 66045 USA. Texas A&M Univ, College Stn, TX 77843 USA. Frederick L Hovde Dean Coll Sci, Frederick, MD USA. Purdue Univ, W Lafayette, IN 47907 USA. Duke Univ, Durham, NC 27706 USA. Tulane Univ, Sch Sci & Engn, New Orleans, LA 70118 USA. Weill Cornell Med Coll, TMHRI, Dept Syst Med & Bioengn, New York, NY USA. Cornell Univ, Ithaca, NY 14853 USA. Harvard Univ, Sch Med, HCNR Ctr Bioinformat, Cambridge, MA 02138 USA. Columbia Univ, Dept Biomed Engn, New York, NY 10027 USA. Howard Hughes Med Inst, Chevy Chase, MD USA. Univ So Maine, Portland, ME 04103 USA. SUNY Buffalo, Dept Comp Sci & Engn, Buffalo, NY 14260 USA. Univ Calif Santa Barbara, Coll Engn, Santa Barbara, CA 93106 USA. Free Univ Berlin, Berlin, Germany. Univ Henri Poincare, Nancy, France. Duke Univ, Med Ctr, Durham, NC USA. Case Western Reserve Univ, Dept Elect Engn & Comp Sci, Cleveland, OH 44106 USA. Univ Delaware, Dept Comp & Informat Sci, Newark, DE 19716 USA. Queens Univ, Kingston, ON, Canada. Carnegie Mellon Univ, Dept Biol Sci, Pittsburgh, PA 15213 USA. Carnegie Mellon Univ, Lane Ctr Computat Biol, Pittsburgh, PA 15213 USA. Mines ParisTech, Ctr Computat Biol, Paris, France. Inst Curie, Lab Bioinformat & Computat Syst Biol Canc, F-75231 Paris, France. City Univ Hong Kong, Dept Comp Sci, Hong Kong, Hong Kong, Peoples R China. Univ Montreal, Montreal Gen Hosp, Montreal, PQ, Canada. NR 0 TC 0 Z9 0 U1 0 U2 10 PU IEEE COMPUTER SOC PI LOS ALAMITOS PA 10662 LOS VAQUEROS CIRCLE, PO BOX 3014, LOS ALAMITOS, CA 90720-1314 USA SN 1545-5963 J9 IEEE ACM T COMPUT BI JI IEEE-ACM Trans. Comput. Biol. Bioinform. PD NOV-DEC PY 2012 VL 9 IS 6 BP 1553 EP 1557 PG 5 WC Biochemical Research Methods; Computer Science, Interdisciplinary Applications; Mathematics, Interdisciplinary Applications; Statistics & Probability SC Biochemistry & Molecular Biology; Computer Science; Mathematics GA 057JD UT WOS:000312558400001 ER PT J AU Sargsyan, K Safta, C Debusschere, B Najm, H AF Sargsyan, Khachik Safta, Cosmin Debusschere, Bert Najm, Habib TI Multiparameter Spectral Representation of Noise-Induced Competence in Bacillus Subtilis SO IEEE-ACM TRANSACTIONS ON COMPUTATIONAL BIOLOGY AND BIOINFORMATICS LA English DT Article DE Approximation; spectral methods; probability and statistics ID COUPLED CHEMICAL-REACTIONS; SENSITIVITY-ANALYSIS; STOCHASTIC SIMULATION; SYSTEMS; DIFFERENTIATION; DYNAMICS; CHAOS AB In this work, the problem of representing a stochastic forward model output with respect to a large number of input parameters is considered. The methodology is applied to a stochastic reaction network of competence dynamics in Bacillus subtilis bacterium. In particular, the dependence of the competence state on rate constants of underlying reactions is investigated. We base our methodology on Polynomial Chaos (PC) spectral expansions that allow effective propagation of input parameter uncertainties to outputs of interest. Given a number of forward model training runs at sampled input parameter values, the PC modes are estimated using a Bayesian framework. As an outcome, these PC modes are described with posterior probability distributions. The resulting expansion can be regarded as an uncertain response function and can further be used as a computationally inexpensive surrogate instead of the original reaction model for subsequent analyses such as calibration or optimization studies. Furthermore, the methodology is enhanced with a classification-based mixture PC formulation that overcomes the difficulties associated with representing potentially nonsmooth input-output relationships. Finally, the global sensitivity analysis based on the multiparameter spectral representation of an observable of interest provides biological insight and reveals the most important reactions and their couplings for the competence dynamics. C1 [Sargsyan, Khachik; Safta, Cosmin; Debusschere, Bert; Najm, Habib] Sandia Natl Labs, Livermore, CA 94550 USA. RP Sargsyan, K (reprint author), Sandia Natl Labs, 7011 E Ave,MS 9051, Livermore, CA 94550 USA. EM ksargsy@sandia.gov; csafta@sandia.gov; bjdebus@sandia.gov; hnnajm@sandia.gov FU US Department of Energy (DOE) Office of Science through the Applied Mathematics program in the Office of Advanced Scientific Computing Research (ASCR) [07-012783]; US Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported by the US Department of Energy (DOE) Office of Science through the Applied Mathematics program in the Office of Advanced Scientific Computing Research (ASCR) under contract 07-012783 with Sandia National Laboratories. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the US Department of Energy's National Nuclear Security Administration under contract No. DE-AC04-94AL85000. NR 33 TC 3 Z9 3 U1 0 U2 7 PU IEEE COMPUTER SOC PI LOS ALAMITOS PA 10662 LOS VAQUEROS CIRCLE, PO BOX 3014, LOS ALAMITOS, CA 90720-1314 USA SN 1545-5963 EI 1557-9964 J9 IEEE ACM T COMPUT BI JI IEEE-ACM Trans. Comput. Biol. Bioinform. PD NOV-DEC PY 2012 VL 9 IS 6 BP 1709 EP 1723 DI 10.1109/TCBB.2012.107 PG 15 WC Biochemical Research Methods; Computer Science, Interdisciplinary Applications; Mathematics, Interdisciplinary Applications; Statistics & Probability SC Biochemistry & Molecular Biology; Computer Science; Mathematics GA 057JD UT WOS:000312558400015 PM 22868681 ER PT J AU Goodall, JR Mansmann, F Gerth, J AF Goodall, John R. Mansmann, Florian Gerth, John TI Computer Network Visualization SO IEEE NETWORK LA English DT Editorial Material C1 [Goodall, John R.] Oak Ridge Natl Lab, Visual Analyt Res Team, Oak Ridge, TN USA. [Mansmann, Florian] Univ Konstanz, Res Project Network Secur, Constance, Germany. [Gerth, John] Stanford Univ, Dept Elect Engn, Stanford, CA 94305 USA. [Gerth, John] Stanford Univ, Dept Comp Sci, Stanford, CA 94305 USA. [Mansmann, Florian] Univ Konstanz, Res Project Geoinformat, Constance, Germany. RP Goodall, JR (reprint author), Oak Ridge Natl Lab, Visual Analyt Res Team, Oak Ridge, TN USA. EM jgoodall@ornl.gov; Florian.Mansmann@uni-konstanz.de; gerth@graphics.stanford.edu NR 0 TC 0 Z9 0 U1 0 U2 7 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0890-8044 J9 IEEE NETWORK JI IEEE Netw. PD NOV-DEC PY 2012 VL 26 IS 6 BP 4 EP 5 DI 10.1109/MNET.2012.6375883 PG 2 WC Computer Science, Hardware & Architecture; Computer Science, Information Systems; Engineering, Electrical & Electronic; Telecommunications SC Computer Science; Engineering; Telecommunications GA 056BF UT WOS:000312461200002 ER PT J AU Zhang, Z Hwang, JY Ning, M Li, X AF Zhang, Zheng Hwang, Jiann-Yang Ning, Ming Li, Xuan TI Field ionization effect on hydrogen adsorption over TiO2-coated activated carbon SO INTERNATIONAL JOURNAL OF HYDROGEN ENERGY LA English DT Article DE Hydrogen adsorption; TiO2-coated carbon; Electric field; Polarization; Ionization ID ROOM-TEMPERATURE; STORAGE; NANOTUBES; SPILLOVER; GRAPHITE; SURFACE; SYSTEM AB Behaviors of hydrogen adsorption over TiO2-coated activated carbon under various electric potentials were studied. TiO2 particles were introduced onto carbon via the hydrolysis of TiCl4 in acid solution. The results showed that the hydrogen adsorption first increased and then decreased with the increase of electric field. The improved storage was due to a stronger interaction between charged carbon surface and polarized hydrogen molecule caused by field induced polarization of TiO2 coating. When the electric field was sufficient to cause considerable ionization of hydrogen, the decrease of hydrogen adsorption occurred. The electricity detected at 3000 V was a sign of ionization of hydrogen. The DFT calculations showed a much stronger binding between TiO2-doped coronene and hydrogen molecule under an electric field, which is consistent with our experimental observations. Copyright (C) 2012, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved. C1 [Zhang, Zheng; Hwang, Jiann-Yang] Michigan Technol Univ, Dept Mat Sci & Engn, Houghton, MI 49931 USA. [Zhang, Zheng] Michigan Technol Univ, Dept Civil & Environm Engn, Houghton, MI 49931 USA. [Ning, Ming] Brookhaven Natl Lab, Upton, NY 11973 USA. [Li, Xuan] Natl Inst Clean & Low Carbon Energy, Beijing 102209, Peoples R China. RP Hwang, JY (reprint author), Michigan Technol Univ, Dept Mat Sci & Engn, Houghton, MI 49931 USA. EM jhwang@mtu.edu FU U.S. Department of Energy's Hydrogen Program [DE-FG36-05GO15003] FX This work was supported by the U.S. Department of Energy's Hydrogen Program, under Award Number DE-FG36-05GO15003. NR 29 TC 6 Z9 8 U1 1 U2 32 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-3199 J9 INT J HYDROGEN ENERG JI Int. J. Hydrog. Energy PD NOV PY 2012 VL 37 IS 21 BP 16018 EP 16024 DI 10.1016/j.ijhydene.2012.08.044 PG 7 WC Chemistry, Physical; Electrochemistry; Energy & Fuels SC Chemistry; Electrochemistry; Energy & Fuels GA 038TK UT WOS:000311196800022 ER PT J AU Michler, T San Marchi, C Naumann, J Weber, S Martin, M AF Michler, Thorsten San Marchi, Chris Naumann, Joerg Weber, Sebastian Martin, Mauro TI Hydrogen environment embrittlement of stable austenitic steels SO INTERNATIONAL JOURNAL OF HYDROGEN ENERGY LA English DT Article DE Hydrogen environment embrittlement; Austenitic stainless steel; Martensitic transformation; Incoloy DS; TWIP; Hadfield ID STACKING-FAULT ENERGY; HIGH-PRESSURE HYDROGEN; STAINLESS-STEELS; LOW-TEMPERATURES; DISLOCATION-STRUCTURES; INDUCED PLASTICITY; ELECTRON-STRUCTURE; STRAIN AMPLITUDE; FEMNAL ALLOYS; DEFORMATION AB Seven stable austenitic steels (stable with respect to gamma -> alpha' transformation at room temperature) of different alloy compositions (18Cr-12.5Ni, 18Cr-35Ni, 18Cr-8Ni-6Mn -0.25N, 0.6C-23Mn, 1.3C-12Mn, 1C-31Mn-9Al, 18Cr-19Mn-0.8N) were tensile tested in high-pressure hydrogen atmosphere to assess the role of austenite stability on hydrogen environment embrittlement (HEE). The influence of hydrogen on tensile ductility was small in steels that are believed to have a high initial portion of dislocation cross slip (18Cr -12.5Ni, 18Cr-35Ni, 18Cr-8Ni-6Mn-0.25N), while the effects of hydrogen were significantly greater in steels with other primary deformation modes (planar slip in 18Cr-19Mn -0.8N and 1C-31Mn-9A1 or mechanical twinning in 0.6C-23Mn and 1.3C-12Mn) despite comparable austenite stability at the given test conditions. It appears that initial deformation mode is one important parameter controlling susceptibility to HEE and that martensitic transformation is not a sufficient explanation for HEE of austenitic steels. Copyright (C) 2012, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved. C1 [Michler, Thorsten] Adam Opel AG, D-65423 Russelsheim, Germany. [San Marchi, Chris] Sandia Natl Labs, Livermore, CA 94550 USA. [Naumann, Joerg] BMW AG, D-80788 Munich, Germany. [Weber, Sebastian] Helmholtz Ctr Berlin Mat & Energy GmbH, D-14109 Berlin, Germany. [Weber, Sebastian; Martin, Mauro] Ruhr Univ Bochum, Inst Mat, Chair Mat Technol, D-44780 Bochum, Germany. RP Michler, T (reprint author), Adam Opel AG, D-65423 Russelsheim, Germany. EM thorsten.dr.michler@de.opel.com; cwsanma@sandia.gov; joerg.naumann@bmw.de; sebastian.weber@helmholz-berlin.de; martin@wtech.rub.de OI San Marchi, Christopher/0000-0002-0862-8607; Martin, Mauro/0000-0001-8389-3067 FU German Bundesministerium fur Wirtschaft und Technologie [0327802A, 0327802D] FX This work was partly funded by the German Bundesministerium fur Wirtschaft und Technologie under contract numbers 0327802A and 0327802D. NR 72 TC 36 Z9 38 U1 6 U2 62 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-3199 EI 1879-3487 J9 INT J HYDROGEN ENERG JI Int. J. Hydrog. Energy PD NOV PY 2012 VL 37 IS 21 BP 16231 EP 16246 DI 10.1016/j.ijhydene.2012.08.071 PG 16 WC Chemistry, Physical; Electrochemistry; Energy & Fuels SC Chemistry; Electrochemistry; Energy & Fuels GA 038TK UT WOS:000311196800042 ER PT J AU Flich, J Pakin, S Stunkel, C AF Flich, Jose Pakin, Scott Stunkel, Craig TI Special issue on Communication Architectures for Scalable Systems SO JOURNAL OF PARALLEL AND DISTRIBUTED COMPUTING LA English DT Editorial Material C1 [Flich, Jose] Univ Politecn Valencia, Valencia 46020, Spain. [Pakin, Scott] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Flich, J (reprint author), Univ Politecn Valencia, Camino de Vera S-N, Valencia 46020, Spain. EM jflich@disca.upv.es OI Pakin, Scott/0000-0002-5220-1985 NR 0 TC 0 Z9 0 U1 0 U2 0 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0743-7315 J9 J PARALLEL DISTR COM JI J. Parallel Distrib. Comput. PD NOV PY 2012 VL 72 IS 11 SI SI BP 1399 EP 1400 DI 10.1016/j.jpdc.2012.05.007 PG 2 WC Computer Science, Theory & Methods SC Computer Science GA 010KF UT WOS:000309092600001 ER PT J AU Yu, WK Que, XY Tipparaju, V Vetter, JS AF Yu, Weikuan Que, Xinyu Tipparaju, Vinod Vetter, Jeffrey S. TI HiCOO: Hierarchical cooperation for scalable communication in Global Address Space programming models on Cray XT systems SO JOURNAL OF PARALLEL AND DISTRIBUTED COMPUTING LA English DT Article DE GAS; ARMCI; Multicore; Multinode; Virtual Topology; Contention ID INTERCONNECTION NETWORKS; PERFORMANCE AB Global Address Space (GAS) programming models enable a convenient, shared-memory style addressing model. Typically this is realized through one-sided operations that can enable asynchronous communication and data movement. With the size of petascale systems reaching 10,000s of nodes and 100,000s of cores, the underlying runtime systems face critical challenges in (1) scalably managing resources (such as memory for communication buffers), and (2) gracefully handling unpredictable communication patterns and any associated contention. For any solution that addresses these resource scalability challenges, equally important is the need to maintain the performance of GAS programming models. In this paper, we describe a Hierarchical COOperation (HiCOO) architecture for scalable communication in GAS programming models. HiCOO formulates a cooperative communication architecture: with inter-node cooperation amongst multiple nodes (a.k.a multinode) and hierarchical cooperation among multinodes that are arranged in various virtual topologies. We have implemented HiCOO for a popular GAS runtime library, Aggregate Remote Memory Copy Interface (ARMCI). By extensively evaluating different virtual topologies in HiCOO in terms of their impact to memory, scalability, network contention, and application performance, we identify MFCG as the most suitable virtual topology. The resulting HiCOO architecture is able to realize scalable resource management and achieve resilience to network contention, while at the same time maintaining or enhancing the performance of scientific applications. In one case, it reduces the total execution time of an NWChem application by 52%. (C) 2012 Elsevier Inc. All rights reserved. C1 [Yu, Weikuan; Que, Xinyu] Auburn Univ, Dept Comp Sci, Auburn, AL 36849 USA. [Tipparaju, Vinod; Vetter, Jeffrey S.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Yu, WK (reprint author), Auburn Univ, Dept Comp Sci, Auburn, AL 36849 USA. EM wkyu@auburn.edu; xque@auburn.edu; tipparajuv@gmail.com; vetter@ornl.gov RI Que, Xinyu/B-1721-2014 FU NSF [CNS-1059376]; UT-Battelle grant [UT-B-4000087151]; National Center for Computational Sciences; Office of Science of the US Department of Energy [DE-AC05-00OR22725] FX This work was funded in part by NSF award CNS-1059376, UT-Battelle grant (UT-B-4000087151), and National Center for Computational Sciences. This research used resources of the National Center for Computational Sciences at Oak Ridge National Laboratory, which is supported by the Office of Science of the US Department of Energy under Contract No. DE-AC05-00OR22725. NR 28 TC 0 Z9 0 U1 0 U2 7 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0743-7315 J9 J PARALLEL DISTR COM JI J. Parallel Distrib. Comput. PD NOV PY 2012 VL 72 IS 11 SI SI BP 1481 EP 1492 DI 10.1016/j.jpdc.2012.01.022 PG 12 WC Computer Science, Theory & Methods SC Computer Science GA 010KF UT WOS:000309092600010 ER PT J AU Kong, LG Uedono, A Smith, SV Yamashita, Y Chironi, I AF Kong, Linggen Uedono, Akira Smith, Suzanne V. Yamashita, Yukihiro Chironi, Ilkay TI Synthesis of silica nanoparticles using oil-in-water emulsion and the porosity analysis SO JOURNAL OF SOL-GEL SCIENCE AND TECHNOLOGY LA English DT Article DE Silica nanoparticles; Sol-gel; Porosity; PALS ID ANNIHILATION LIFETIME SPECTROSCOPY; POSITRON-ANNIHILATION; MESOPOROUS SILICA; PORE-SIZE; BIOSENSING APPLICATIONS; PHOTODYNAMIC THERAPY; DRUG-DELIVERY; THIN-FILMS; SYSTEM; PROBES AB A set of silica particles was synthesized in oil-in-water emulsion with particle diameters ranging from similar to 42 nm to similar to 115 nm approximately. The porosity of the nanoparticles was analyzed using conventional nitrogen sorption and positron annihilation lifetime spectroscopy (PALS) techniques. The isotherm obtained using nitrogen sorption indicated that the particles were 'non-porous', however fitting data with Density Functional Theory model revealed a low concentration pore with diameters from 1.4 nm to 1.7 nm. The pore size was independent of the particle size. In contrast, analysis with PALS revealed a single pore size of similar to 0.6 nm present in all samples. Difference in results obtained for micropores < 4 nm diameter is proposed to be dependent on models used and sample conditions for analysis. C1 [Kong, Linggen; Chironi, Ilkay] Australian Nucl Sci & Technol Org, Inst Mat Engn, Kirrawee, NSW 2232, Australia. [Uedono, Akira; Yamashita, Yukihiro] Univ Tsukuba, Div Appl Phys, Fac Pure & Appl Sci, Tsukuba, Ibaraki 3058573, Japan. [Smith, Suzanne V.] Brookhaven Natl Lab, Collider Accelerator Dept, Upton, NY 11973 USA. [Smith, Suzanne V.] Australian Natl Univ, Ctr Excellence Antimatter Matter Studies, Canberra, ACT 0200, Australia. RP Kong, LG (reprint author), Australian Nucl Sci & Technol Org, Inst Mat Engn, Locked Bag 2001, Kirrawee, NSW 2232, Australia. EM lnk@ansto.gov.au NR 43 TC 1 Z9 1 U1 5 U2 18 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0928-0707 J9 J SOL-GEL SCI TECHN JI J. Sol-Gel Sci. Technol. PD NOV PY 2012 VL 64 IS 2 BP 309 EP 314 DI 10.1007/s10971-012-2859-7 PG 6 WC Materials Science, Ceramics SC Materials Science GA 057SN UT WOS:000312584400007 ER PT J AU Clapsaddle, BJ Neumann, B Wittstock, A Sprehn, DW Gash, AE Satcher, JH Simpson, RL Baumer, M AF Clapsaddle, Brady J. Neumann, Bjoern Wittstock, Arne Sprehn, David W. Gash, Alexander E. Satcher, Joe H., Jr. Simpson, Randall L. Baeumer, Marcus TI A sol-gel methodology for the preparation of lanthanide-oxide aerogels: preparation and characterization SO JOURNAL OF SOL-GEL SCIENCE AND TECHNOLOGY LA English DT Article DE Aerogels; Catalysts; Lanthanide oxides; Lanthanide oxychlorides; Rare-earth oxide aerogel ID RARE-EARTH-OXIDES; HIGH-ENERGY DIFFRACTION; THIN-FILMS; ELECTRICAL-PROPERTIES; CATALYTIC-PROPERTIES; LOW-TEMPERATURE; ROUTE; NANOPARTICLES; TRANSITION; MONOLITHS AB Lanthanide oxide-based aerogels were synthesized employing the so-called epoxide addition sol-gel method already successfully applied for main- and transition metal oxide aerogels. Using chlorides and nitrates as precursors, our aim was to test the transferability of this robust sol-gel methodology to the entire lanthanide series. By adding the proton scavenging organic epoxide, propylene oxide, to hydrated lanthanide trichloride dissolved in ethanol or methanol, uniform monolithic alcogels were obtained. Subsequent processing in supercritical CO2 resulted in monolithic aerogels. No gelling process could be induced by using nitrates, in contrast to previous results with iron oxide or alumina aerogels. All materials were characterized by nitrogen adsorption/desorption analysis, transmission electron microscopy, and powder X-ray diffraction. With the exception of cerium, for which fractions of crystalline CeO2 were found already in the as-prepared material, XRD analysis revealed that the other materials were mainly amorphous. Subsequent heat treatment of the aerogels above 650 A degrees C resulted in nanocrystalline phases for all aerogel materials. However, except for ceria, more detailed TEM and XRD studies provided evidence that crystalline oxychloride phases are formed in addition to fractions of oxide phases. The trends and possible explanations are discussed in this contribution. A sol-gel methodology using organic epoxides as proton scavengers has been used to synthesize oxide aerogels of the entire lanthanide series. As precursors, nitrates and chlorides were used but only in the latter case, gelation set in. After supercritical drying, aerogels with high surface areas and mesoporous, nanoparticulate structures were obtained. Further characterization revealed that cerium plays a special role, since it contained crystalline CeO2 fractions already before calcination. After calcination it was the only material consisting of a pure oxide phase. The syntheses with the other lanthanides resulted in mixtures with varying fractions of crystalline oxychlorides in addition to an oxide phase. The trends and possible explanations are discussed in this contribution.A sol-gel methodology using organic epoxides as proton scavengers has been used to synthesize oxide aerogels of the entire lanthanide series. As precursors, nitrates and chlorides were used but only in the latter case, gelation set in. After supercritical drying, aerogels with high surface areas and mesoporous, nanoparticulate structures were obtained. Further characterization revealed that cerium plays a special role, since it contained crystalline CeO2 fractions already before calcination. After calcination it was the only material consisting of a pure oxide phase. The syntheses with the other lanthanides resulted in mixtures with varying fractions of crystalline oxychlorides in addition to an oxide phase. The trends and possible explanations are discussed in this contribution. C1 [Clapsaddle, Brady J.; Neumann, Bjoern; Sprehn, David W.; Gash, Alexander E.; Satcher, Joe H., Jr.; Simpson, Randall L.] Lawrence Livermore Natl Lab, Div Chem & Chem Engn, Chem & Mat Sci Directorate, Livermore, CA 94550 USA. [Neumann, Bjoern; Wittstock, Arne; Baeumer, Marcus] Univ Bremen, Inst Appl & Phys Chem, D-28359 Bremen, Germany. RP Gash, AE (reprint author), Lawrence Livermore Natl Lab, Div Chem & Chem Engn, Chem & Mat Sci Directorate, Livermore, CA 94550 USA. EM gash2@llnl.gov RI Baumer, Marcus/S-5441-2016 OI Baumer, Marcus/0000-0002-8620-1764 FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344, LLNL-JRNL-562011]; Telekom Stiftung FX This work performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344, reference number LLNL-JRNL-562011. The authors would like to thank Christopher Chervin (LLNL) and Thorsten Gesing (University Bremen) for helpful analysis of the X-ray diffraction data. Special thanks go to Morris Wang and Jennifer S. Harper for TEM and EELS analyses and Cheng Saw for PXRD measurements. BN is grateful to the Telekom Stiftung for a stipend. NR 50 TC 10 Z9 11 U1 6 U2 140 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0928-0707 J9 J SOL-GEL SCI TECHN JI J. Sol-Gel Sci. Technol. PD NOV PY 2012 VL 64 IS 2 BP 381 EP 389 DI 10.1007/s10971-012-2868-6 PG 9 WC Materials Science, Ceramics SC Materials Science GA 057SN UT WOS:000312584400016 ER PT J AU Scullard, CR AF Scullard, Christian R. TI The computation of bond percolation critical polynomials by the deletion-contraction algorithm SO JOURNAL OF STATISTICAL MECHANICS-THEORY AND EXPERIMENT LA English DT Article DE rigorous results in statistical mechanics; solvable lattice models ID ARCHIMEDEAN LATTICES; KAGOME LATTICE; 2 DIMENSIONS; THRESHOLDS; BOUNDS; MODELS AB Although every exactly known bond percolation critical threshold is the root in [0, 1] of a lattice-dependent polynomial, it has recently been shown that the notion of a critical polynomial can be extended to any periodic lattice. The polynomial is computed on a finite subgraph, called the base, of an infinite lattice. For any problem with exactly known solution, the prediction of the bond threshold is always correct for any base containing an arbitrary number of unit cells. For unsolved problems, the polynomial is referred to as the generalized critical polynomial and provides an approximation that becomes more accurate with increasing number of bonds in the base, appearing to approach the exact answer. The polynomials are computed using the deletion-contraction algorithm, which quickly becomes intractable by hand for more than about 18 bonds. Here, I present generalized critical polynomials calculated with a computer program for bases of up to 36 bonds for all the unsolved Archimedean lattices, except the kagome lattice, which was considered in an earlier work. The polynomial estimates are generally within 10(-5)-10(-7) of the numerical values, but the prediction for the (4, 8(2)) lattice, though not exact, is not ruled out by simulations. C1 Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Scullard, CR (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM scullard1@llnl.gov FU US Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 37 TC 2 Z9 2 U1 0 U2 3 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1742-5468 J9 J STAT MECH-THEORY E JI J. Stat. Mech.-Theory Exp. PD NOV PY 2012 AR P11011 DI 10.1088/1742-5468/2012/11/P11011 PG 23 WC Mechanics; Physics, Mathematical SC Mechanics; Physics GA 051CP UT WOS:000312102500015 ER PT J AU Adams, WP Henry, SM AF Adams, Warren P. Henry, Stephen M. TI Base-2 Expansions for Linearizing Products of Functions of Discrete Variables SO OPERATIONS RESEARCH LA English DT Article ID SUPERIOR REPRESENTATION METHOD; GLOBAL OPTIMIZATION; DESIGN AB This paper presents an approach for representing functions of discrete variables, and their products, using logarithmic numbers of binary variables. Given a univariate function whose domain consists of n distinct values, it begins by employing a base-2 expansion to express the function in terms of the ceiling of log(2) n binary and n continuous variables, using linear restrictions to equate the functional values with the possible binary realizations. The representation of the product of such a function with a nonnegative variable is handled via an appropriate scaling of the linear restrictions. Products of m functions are treated in an inductive manner from i = 2 to m, where each step i uses such a scaling to express the product of function i and a nonnegative variable denoting a translated version of the product of functions 1 through i - 1 as a newly defined variable. The resulting representations, both in terms of one function and many, are important for reformulating general discrete variables as binary, and also for linearizing mixed-integer generalized geometric and discrete nonlinear programs, where it is desired to economize on the number of binary variables. The approach provides insight into, improves upon, and subsumes related linearization methods for products of functions of discrete variables. Subject classifications: programming: integer, nonlinear, theory: Area of review: Optimization. History: Received January 2011; revision received July 2011; accepted October 2011. Published online in Articles in Advance November 20, 2012. C1 [Adams, Warren P.] Clemson Univ, Dept Math Sci, Clemson, SC 29634 USA. [Henry, Stephen M.] Sandia Natl Labs, Syst Readiness & Sustainment Technol Grp, Albuquerque, NM 87123 USA. RP Adams, WP (reprint author), Clemson Univ, Dept Math Sci, Clemson, SC 29634 USA. EM wadams@clemson.edu; smhenry@sandia.gov FU National Science Foundation [CMMI-0968909] FX The authors thank two anonymous referees for their insightful comments and suggestions. The authors are grateful to the National Science Foundation for partially supporting this research [Grant CMMI-0968909]. NR 16 TC 6 Z9 6 U1 1 U2 10 PU INFORMS PI CATONSVILLE PA 5521 RESEARCH PARK DR, SUITE 200, CATONSVILLE, MD 21228 USA SN 0030-364X J9 OPER RES JI Oper. Res. PD NOV-DEC PY 2012 VL 60 IS 6 BP 1477 EP 1490 DI 10.1287/opre.1120.1106 PG 14 WC Management; Operations Research & Management Science SC Business & Economics; Operations Research & Management Science GA 056DO UT WOS:000312468800013 ER PT J AU Pahlevan, N Garrett, AJ Gerace, AD Schott, JR AF Pahlevan, Nima Garrett, Alfred J. Gerace, Aaron D. Schott, John R. TI Integrating Landsat-7 Imagery with Physics-based Models for Quantitative Mapping of Coastal Waters near River Discharges SO PHOTOGRAMMETRIC ENGINEERING AND REMOTE SENSING LA English DT Article ID SUSPENDED SEDIMENT; TURBID WATERS; REMOTE; CIRCULATION; LAKE; CALIBRATION; QUALITY; FIELD AB Remote sensing has traditionally been used to retrieve water constituents by establishing a relationship between in situ measured quantities and image-derived products. Motivated by the dramatically improved potential of the Landsat Data Continuity Mission (LDCM), this paper describes a different approach for water constituent retrieval where both thermal and visible spectral bands of the Enhanced Thematic Mapper Plus (ETM+) instrument on board Landsat-7 are utilized. In this effort, Landsat data is integrated with a 3D hydrodynamic model to obtain profiles of particles and dissolved matter in the near shore zone in the vicinity of two river discharges. The procedure is based upon performing many hydrodynamic simulations by adjusting input environmental/physical variables and generating Look-Up-Tables (LUTs). The best match, obtained using optimization, demonstrated an average root-mean-squared-error (RMSE) of 0.68 percent, i.e., 0.0068 reflectance units, calculated over the two river plumes. It is concluded that calibrating a physics-based model using the Landsat-7 imagery can provide a more lucid insight into the dynamics of spatially non-uniform waters. C1 [Pahlevan, Nima] Univ Massachusetts, Dept Environm Earth & Ocean Sci, Boston, MA 02125 USA. [Pahlevan, Nima; Gerace, Aaron D.; Schott, John R.] Rochester Inst Technol, Chester F Carlson Ctr Imaging Sci, Rochester, NY 14623 USA. [Garrett, Alfred J.] Savannah River Natl Lab, Aiken, SC 29808 USA. RP Pahlevan, N (reprint author), Univ Massachusetts, Dept Environm Earth & Ocean Sci, 100 Morrissey Blvd, Boston, MA 02125 USA. EM nima.pahlevan@umb.edu RI Pahlevan, Nima/L-7746-2014 OI Pahlevan, Nima/0000-0002-5454-5212 FU United State Geological Survey (USGS) [06CRCN0024] FX This work was funded by the United State Geological Survey (USGS) under the contract No. 06CRCN0024. The authors appreciate the staff at the Research Computing (RC) center of Rh for facilitating the computational burden of this study. We also would like to thank Mrs. Nina Gibson Raqueno and Dr. Rolando Raqueno with the Digital Imaging and Remote Sensing Laboratory (Elms) for their assistance and the previous research efforts in similar studies conducted at RIT. It should also be noted that the content of this paper does not represent the views or policies of the Department of Interior, nor does mention of the trade names, commercial products or organizations imply endorsement by the US Government. NR 37 TC 3 Z9 3 U1 2 U2 15 PU AMER SOC PHOTOGRAMMETRY PI BETHESDA PA 5410 GROSVENOR LANE SUITE 210, BETHESDA, MD 20814-2160 USA SN 0099-1112 J9 PHOTOGRAMM ENG REM S JI Photogramm. Eng. Remote Sens. PD NOV PY 2012 VL 78 IS 11 BP 1163 EP 1174 PG 12 WC Geography, Physical; Geosciences, Multidisciplinary; Remote Sensing; Imaging Science & Photographic Technology SC Physical Geography; Geology; Remote Sensing; Imaging Science & Photographic Technology GA 036VC UT WOS:000311059300008 ER PT J AU Ling, Y Wagner, JL Beresh, SJ Kearney, SP Balachandar, S AF Ling, Y. Wagner, J. L. Beresh, S. J. Kearney, S. P. Balachandar, S. TI Interaction of a planar shock wave with a dense particle curtain: Modeling and experiments SO PHYSICS OF FLUIDS LA English DT Article DE computational fluid dynamics; drag; flow instability; flow simulation; hydrodynamics; shock wave effects; two-phase flow ID GAS-FLUIDIZED BEDS; UNSTEADY CONTRIBUTIONS; NUMERICAL-SIMULATION; COMPRESSIBLE FLOWS; PARTICULATE FLOWS; SPHERE; DRAG; MOTION; FORCE; CYLINDERS AB The interaction of a planar shock wave with a dense particle curtain is investigated through modeling and experiments. The physics in the interaction between a shock wave with a dense gas-particle mixture is markedly differently from that with a dilute mixture. Following the passage of the shock wave, the dense particle curtain expands rapidly as it propagates downstream and pressures equilibrate throughout the flow field. In the simulations, the particles are viewed as point-particles and are traced in a Lagrangian framework. A physics-based model is then developed to account for interphase coupling. Compared to the standard drag law, four major improvements are made in the present interphase coupling model to take into account: (1) unsteady force contributions to particle force; (2) effect of compressibility on hydrodynamic forces; (3) effect of particle volume fraction on hydrodynamic forces; (4) effect of inter-particle collision. The complex behavior of the dense particle curtain is due to the interplay between two-way coupling, finite particle inertia, and unsteady forces. Incorporation of these effects through significant modeling improvements is essential for the simulation results to agree well with the experimental data. As a result of the large pressure gradient inside the particle curtain, the unsteady forces remain significant for a long time compared to the quasi-steady force and greatly influence the particle curtain motion. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4768815] C1 [Ling, Y.; Balachandar, S.] Univ Florida, Dept Mech & Aerosp Engn, Gainesville, FL 32611 USA. [Wagner, J. L.; Beresh, S. J.; Kearney, S. P.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Ling, Y (reprint author), Univ Florida, Dept Mech & Aerosp Engn, Gainesville, FL 32611 USA. EM yueling@ufl.edu FU AFOSR [FA 9550-10-1-0309]; Sandia National Laboratories; United States Department of Energy; internal Laboratory Directed Research and Development (LDRD) grant; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors would like to acknowledge support from AFOSR (Grant No. FA 9550-10-1-0309). The authors also thank Brian Pruett and Elton Wright for their assistance with the experiments. The experiments were supported by Sandia National Laboratories and the United States Department of Energy with an internal Laboratory Directed Research and Development (LDRD) grant. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration (Contract No. DE-AC04-94AL85000). NR 58 TC 19 Z9 19 U1 7 U2 39 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 1070-6631 J9 PHYS FLUIDS JI Phys. Fluids PD NOV PY 2012 VL 24 IS 11 AR 113301 DI 10.1063/1.4768815 PG 30 WC Mechanics; Physics, Fluids & Plasmas SC Mechanics; Physics GA 050DO UT WOS:000312033200016 ER PT J AU Higashi, M Horblyuk, R North, M Graziano, D Macal, C Sarawate, C Kruzikas, D Collier, N AF Higashi, M. Horblyuk, R. North, M. Graziano, D. Macal, C. Sarawate, C. Kruzikas, D. Collier, N. TI AGENT-BASED CARDIOVASCULAR DISEASE MODEL FOR INDIA SO VALUE IN HEALTH LA English DT Meeting Abstract C1 [Higashi, M.] GE Healthcare, Palatine, IL USA. [Horblyuk, R.; Kruzikas, D.] GE Healthcare, Wauwatosa, WI USA. [North, M.; Graziano, D.; Macal, C.; Collier, N.] Argonne Natl Lab, Argonne, IL 60439 USA. [Sarawate, C.] GE Healthcare, Bangalore, Karnataka, India. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 1098-3015 J9 VALUE HEALTH JI Value Health PD NOV PY 2012 VL 15 IS 7 BP A360 EP A360 PG 1 WC Economics; Health Care Sciences & Services; Health Policy & Services SC Business & Economics; Health Care Sciences & Services GA 055JF UT WOS:000312411100442 ER PT J AU Notz, PK Pawlowski, RP Sutherland, JC AF Notz, Patrick K. Pawlowski, Roger P. Sutherland, James C. TI Graph-Based Software Design for Managing Complexity and Enabling Concurrency in Multiphysics PDE Software SO ACM TRANSACTIONS ON MATHEMATICAL SOFTWARE LA English DT Article DE Algorithms; Design; Scientific computing; object-oriented design; multiphysics; task graph ID ALGEBRAIC MULTILEVEL PRECONDITIONER; COMPUTATIONAL FLUID-DYNAMICS; ADVECTIVE-DIFFUSIVE SYSTEMS; FINITE-ELEMENT FORMULATION; KRYLOV METHODS; RESISTIVE MHD; PARALLEL; FRAMEWORK; DIFFERENTIATION; OPTIMIZATION AB Multiphysics simulation software is plagued by complexity stemming from nonlinearly coupled systems of Partial Differential Equations (PDEs). Such software typically supports many models, which may require different transport equations, constitutive laws, and equations of state. Strong coupling and a multiplicity of models leads to complex algorithms (i.e., the properly ordered sequence of steps to assemble a discretized set of coupled PDEs) and rigid software. This work presents a design strategy that shifts focus away from high-level algorithmic concerns to low-level data dependencies. Mathematical expressions are represented as software objects that directly expose data dependencies. The entire system of expressions forms a directed acyclic graph and the high-level assembly algorithm is generated automatically through standard graph algorithms. This approach makes problems with complex dependencies entirely tractable, and removes virtually all logic from the algorithm itself. Changes are highly localized, allowing developers to implement models without detailed understanding of any algorithms (i.e., the overall assembly process). Furthermore, this approach complements existing MPI-based frameworks and can be implemented within them easily. Finally, this approach enables algorithmic parallelization via threads. By exposing dependencies in the algorithm explicitly, thread-based parallelism is implemented through algorithm decomposition, providing a basis for exploiting parallelism independent from domain decomposition approaches. C1 [Notz, Patrick K.] Sandia Natl Labs, Engn Sci Ctr, Albuquerque, NM 87185 USA. [Sutherland, James C.] Univ Utah, Salt Lake City, UT 84112 USA. RP Notz, PK (reprint author), Sandia Natl Labs, Engn Sci Ctr, POB 5800,MS 0836, Albuquerque, NM 87185 USA. EM pknotz@sandia.gov OI Sutherland, James/0000-0002-2955-3472 FU DOE NNSA ASC Integrated Codes effort at Sandia National Laboratories [DE-AC04-94AL85000]; DOE NNSA ASC Algorithms effort; DOE Office of Science AMR program at Sandia National Laboratories [DE-AC04-94AL85000]; National Nuclear Security Administration under the Advanced Simulation and Computing program through DOE Research Grant [DE-NA0000740]; National Science Foundation [PetaApps-0904631]; United States Department of Energy' s National Nuclear Security Administration [DE-AC04-94AL85000] FX P. K. Notz acknowledges support from the DOE NNSA ASC Integrated Codes effort at Sandia National Laboratories under contract DE-AC04-94AL85000. R. P. Pawlowski acknowledges support from the DOE NNSA ASC Algorithms effort and the DOE Office of Science AMR program at Sandia National Laboratories under contract DE-AC04-94AL85000. J. C. Sutherland acknowledges support form the National Nuclear Security Administration under the Advanced Simulation and Computing program through DOE Research Grant DE-NA0000740 and by the National Science Foundation through grant no. PetaApps-0904631. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy' s National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 47 TC 10 Z9 10 U1 0 U2 11 PU ASSOC COMPUTING MACHINERY PI NEW YORK PA 2 PENN PLAZA, STE 701, NEW YORK, NY 10121-0701 USA SN 0098-3500 J9 ACM T MATH SOFTWARE JI ACM Trans. Math. Softw. PD NOV PY 2012 VL 39 IS 1 AR 1 DI 10.1145/2382585.2382586 PG 21 WC Computer Science, Software Engineering; Mathematics, Applied SC Computer Science; Mathematics GA 052PW UT WOS:000312211500001 ER PT J AU Wang, L Lei, HW Ren, SJ Bu, Q Liang, J Wei, Y Liu, YP Lee, GSJ Chen, SL Tang, J Zhang, Q Ruan, R AF Wang, Lu Lei, Hanwu Ren, Shoujie Bu, Quan Liang, Jing Wei, Yi Liu, Yupeng Lee, Guo-Shuh J. Chen, Shulin Tang, Juming Zhang, Qin Ruan, Roger TI Aromatics and phenols from catalytic pyrolysis of Douglas fir pellets in microwave with ZSM-5 as a catalyst SO JOURNAL OF ANALYTICAL AND APPLIED PYROLYSIS LA English DT Article DE Microwave; Catalytic pyrolysis; Douglas fir pellet; ZSM-5; Aromatics; Phenols; GC/MS ID STEP HYDROGENATION-ESTERIFICATION; FIXED-BED REACTOR; BIOMASS PYROLYSIS; BIO-OIL; TEMPERATURE; QUALITY; FUELS; TIME; ACID AB Microwave assisted catalytic pyrolysis was investigated to convert Douglas fir pellets to bio-oils by a ZSM-5 zeolite catalyst. A central composite experimental design (CCD) was used to optimize the catalytic pyrolysis process. The effects of reaction time, temperature and catalyst to biomass ratio on the bio-oil, syngas, and biochar yields were determined. GC/MS analysis results showed that the bio-oil contained a series of important and useful chemical compounds. Phenols, guaiacols, and aromatic hydrocarbons were the most abundant compounds which were about 50-82% in bio-oil depending on the pyrolysis conditions. Comparison between the bio-oils from microwave pyrolysis with and without catalyst showed that the catalyst increased the content of aromatic hydrocarbons and phenols. A reaction pathway was proposed for microwave assisted catalyst pyrolysis of Douglas fir pellets. (C) 2012 Elsevier B.V. All rights reserved. C1 [Wang, Lu; Lei, Hanwu; Ren, Shoujie; Bu, Quan; Liang, Jing; Wei, Yi; Liu, Yupeng; Chen, Shulin; Tang, Juming; Zhang, Qin] Washington State Univ, Dept Biol Syst Engn, Bioprod Sci & Engn Lab, Richland, WA 99354 USA. [Lee, Guo-Shuh J.] Pacific NW Natl Lab, Richland, WA 99354 USA. [Ruan, Roger] Univ Minnesota, Dept Bioprod & Biosyst Engn, St Paul, MN 55108 USA. RP Lei, HW (reprint author), Washington State Univ, Dept Biol Syst Engn, Bioprod Sci & Engn Lab, Richland, WA 99354 USA. EM hlei@tricity.wsu.edu RI ren, shoujie/P-1384-2014; OI Ruan, Roger/0000-0001-8835-2649 FU Office of Research at Washington State University FX This work was supported in partial by the Office of Research at Washington State University. NR 32 TC 17 Z9 18 U1 4 U2 54 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0165-2370 EI 1873-250X J9 J ANAL APPL PYROL JI J. Anal. Appl. Pyrolysis PD NOV PY 2012 VL 98 BP 194 EP 200 DI 10.1016/j.jaap.2012.08.002 PG 7 WC Chemistry, Analytical; Spectroscopy SC Chemistry; Spectroscopy GA 052XB UT WOS:000312232500025 ER PT J AU Font-Ribera, A Miralda-Escude, J Arnau, E Carithers, B Lee, KG Noterdaeme, P Paris, I Petitjean, P Rich, J Rollinde, E Ross, NP Schneider, DP White, M York, DG AF Font-Ribera, Andreu Miralda-Escude, Jordi Arnau, Eduard Carithers, Bill Lee, Khee-Gan Noterdaeme, Pasquier Paris, Isabelle Petitjean, Patrick Rich, James Rollinde, Emmanuel Ross, Nicholas P. Schneider, Donald P. White, Martin York, Donald G. TI The large-scale cross-correlation of Damped Lyman alpha systems with the Lyman alpha forest: first measurements from BOSS SO JOURNAL OF COSMOLOGY AND ASTROPARTICLE PHYSICS LA English DT Article DE redshift surveys; Lyman alpha forest; intergalactic media; galaxy formation ID DIGITAL SKY SURVEY; QUASAR TARGET SELECTION; DARK-MATTER MODEL; LY-ALPHA; DATA RELEASE; LIMIT ABSORBERS; HIGH-REDSHIFT; GALAXIES; ABSORPTION; KINEMATICS AB We present the first measurement of the large-scale cross-correlation of Ly alpha forest absorption and Damped Lyman alpha systems (DLA), using the 9th Data Release of the Baryon Oscillation Spectroscopic Survey (BOSS). The cross-correlation is clearly detected on scales up to 40 h(-1)Mpc and is well fitted by the linear theory prediction of the standard Cold Dark Matter model of structure formation with the expected redshift distortions, confirming its origin in the gravitational evolution of structure. The amplitude of the DLA-Ly alpha cross-correlation depends on only one free parameter, the bias factor of the DLA systems, once the Ly alpha forest bias factors are known from independent Ly alpha forest correlation measurements. We measure the DLA bias factor to be b(D) = (2.17 +/- 0.20)beta(0.22)(F), where the Ly alpha forest redshift distortion parameter beta(F) is expected to be above unity. This bias factor implies a typical host halo mass for DLAs that is much larger than expected in present DLA models, and is reproduced if the DLA cross section scales with halo mass as M-h(alpha), with alpha = 1.1 +/- 0.1 for beta(F) = 1. Matching the observed DLA bias factor and rate of incidence requires that atomic gas remains extended in massive halos over larger areas than predicted in present simulations of galaxy formation, with typical DLA proper sizes larger than 20 kpc in host halos of masses similar to 10(12) M-circle dot. We infer that typical galaxies at z similar or equal to 2 to 3 are surrounded by systems of atomic clouds that are much more extended than the luminous parts of galaxies and contain similar to 10% of the baryons in the host halo. C1 [Font-Ribera, Andreu] Univ Zurich, Inst Theoret Phys, CH-8057 Zurich, Switzerland. [Font-Ribera, Andreu; Carithers, Bill; Ross, Nicholas P.; White, Martin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Miralda-Escude, Jordi] Inst Catalana Recerca & Estudis Avancats, Barcelona, Catalonia, Spain. [Miralda-Escude, Jordi; Arnau, Eduard] Inst Ciencies Cosmos IEEC UB, Barcelona, Catalonia, Spain. [Lee, Khee-Gan] Max Planck Inst Astron, D-69117 Heidelberg, Germany. [Noterdaeme, Pasquier; Paris, Isabelle; Petitjean, Patrick; Rollinde, Emmanuel] Univ Paris 06, Inst Astrophys Paris, F-75014 Paris, France. [Noterdaeme, Pasquier; Paris, Isabelle; Petitjean, Patrick; Rollinde, Emmanuel] CNRS, F-75014 Paris, France. [Paris, Isabelle] Univ Chile, Dept Astron, Santiago, Chile. [Rich, James] CEA, Ctr Saclay, IRFU, F-91191 Gif Sur Yvette, France. [Schneider, Donald P.] Penn State Univ, Dept Astron & Astrophys, University Pk, PA 16802 USA. [Schneider, Donald P.] Penn State Univ, Inst Gravitat & Cosmos, University Pk, PA 16802 USA. [White, Martin] Univ Calif Berkeley, Dept Phys & Astron, Berkeley, CA 94720 USA. [York, Donald G.] Univ Chicago, Dept Astron & Astrophys, Chicago, IL 60637 USA. [York, Donald G.] Univ Chicago, Fermi Inst, Chicago, IL 60637 USA. RP Font-Ribera, A (reprint author), Univ Zurich, Inst Theoret Phys, CH-8057 Zurich, Switzerland. EM font@physik.uzh.ch; miralda@icc.ub.edu RI White, Martin/I-3880-2015; OI White, Martin/0000-0001-9912-5070; Miralda-Escude, Jordi/0000-0002-2316-8370 FU Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; Spanish grants [AYA2009-09745, CSD2007-00060]; Alfred P. Sloan Foundation; National Science Foundation; U.S. Department of Energy Office of Science; SDSS-III Collaboration; University of Arizona; Brazilian Participation Group; Brookhaven National Laboratory; University of Cambridge; Carnegie Mellon University; University of Florida; French Participation Group; German Participation Group; Harvard University; Instituto de Astrofisica de Canarias; Michigan State/Notre Dame/JINA Participation Group; Johns Hopkins University; Lawrence Berkeley National Laboratory; Max Planck Institute for Astrophysics; Max Planck Institute for Extraterrestrial Physics; New Mexico State University; New York University; Ohio State University; Pennsylvania State University; University of Portsmouth; Princeton University; Spanish Participation Group; University of Tokyo; University of Utah; Vanderbilt University; University of Virginia; University of Washington; Yale University FX This research used resources of the National Energy Research Scientific Computing Center (NERSC), which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231, and was also supported by Spanish grants AYA2009-09745 and CSD2007-00060.; Funding for SDSS-III has been provided by the Alfred P. Sloan Foundation, the Participating Institutions, the National Science Foundation, and the U.S. Department of Energy Office of Science. The SDSS-III web site is http://www.sdss3.org/.; SDSS-III is managed by the Astrophysical Research Consortium for the Participating Institutions of the SDSS-III Collaboration including the University of Arizona, the Brazilian Participation Group, Brookhaven National Laboratory, University of Cambridge, Carnegie Mellon University, University of Florida, the French Participation Group, the German Participation Group, Harvard University, the Instituto de Astrofisica de Canarias, the Michigan State/Notre Dame/JINA Participation Group, Johns Hopkins University, Lawrence Berkeley National Laboratory, Max Planck Institute for Astrophysics, Max Planck Institute for Extraterrestrial Physics, New Mexico State University, New York University, Ohio State University, Pennsylvania State University, University of Portsmouth, Princeton University, the Spanish Participation Group, University of Tokyo, University of Utah, Vanderbilt University, University of Virginia, University of Washington, and Yale University. NR 60 TC 57 Z9 57 U1 0 U2 4 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1475-7516 J9 J COSMOL ASTROPART P JI J. Cosmol. Astropart. Phys. PD NOV PY 2012 IS 11 AR 059 DI 10.1088/1475-7516/2012/11/059 PG 42 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 053IA UT WOS:000312263500042 ER PT J AU Scott, P Savage, C Edsjo, J Collaboration, I Abbasi, R Abdou, Y Ackermann, M Adams, J Aguilar, JA Ahlers, M Altmann, D Andeen, K Enberg, JAF Bai, X Baker, M Barwick, SW Baum, V Bay, R Beattie, K Beatty, JJ Bechet, S Tjus, JB Becker, KH Bell, M Benabderrahmane, ML BenZvi, S Berdermann, J Berghaus, P Berley, D Bernardini, E Bertrand, D Besson, DZ Bindig, D Bissok, M Blaufuss, E Blumenthal, J Boersma, DJ Bohm, C Bose, D Boser, S Botner, O Brayeur, L Brown, AM Bruijn, R Brunner, J Buitink, S Caballero-Mora, KS Carson, M Casey, J Casier, M Chirkin, D Christy, B Clevermann, F Cohen, S Cowen, DF Silva, AHC Danninger, M Daughhetee, J Davis, JC De Clercq, C Descamps, F Desiati, P de Vries-Uiterweerd, G DeYoung, T Diaz-Velez, JC Dreyer, J Dumm, JP Dunkman, M Eagan, R Eisch, J Ellsworth, RW Engdegard, O Euler, S Evenson, PA Fadiran, O Fazely, AR Fedynitch, A Feintzeig, J Feusels, T Filimonov, K Finley, C Fischer-Wasels, T Flis, S Franckowiak, A Franke, R Frantzen, K Fuchs, T Gaisser, TK Gallagher, J Gerhardt, L Gladstone, L Glusenkamp, T Goldschmidt, A Goodman, JA Gora, D Grant, D Gross, A Grullon, S Gurtner, M Ha, C Ismail, AH Hallgren, A Halzen, F Hanson, K Heereman, D Heimann, P Heinen, D Helbing, K Hellauer, R Hickford, S Hill, GC Hoffman, KD Hoffmann, R Homeier, A Hoshina, K Huelsnitz, W Hulth, PO Hultqvist, K Hussain, S Ishihara, A Jacobi, E Jacobsen, J Japaridze, GS Jlelati, O Johansson, H Kappes, A Karg, T Karle, A Kiryluk, J Kislat, F Klas, J Klein, SR Kohne, JH Kohnen, G Kolanoski, H Kopke, L Kopper, C Kopper, S Koskinen, DJ Kowalski, M Krasberg, M Kroll, G Kunnen, J Kurahashi, N Kuwabara, T Labare, M Laihem, K Landsman, H Larson, MJ Lauer, R Lesiak-Bzdak, M Lunemann, J Madsen, J Maruyama, R Mase, K Matis, HS McNally, F Meagher, K Merck, M Meszaros, P Meures, T Miarecki, S Middell, E Milke, N Miller, J Mohrmann, L Montaruli, T Morse, R Movit, SM Nahnhauer, R Naumann, U Nowicki, SC Nygren, DR Obertacke, A Odrowski, S Olivas, A Olivo, M O'Murchadha, A Panknin, S Paul, L Pepper, JA de los Heros, CP Pieloth, D Pirk, N Posselt, J Price, PB Przybylski, GT Raedel, L Rawlins, K Redl, P Resconi, E Rhode, W Ribordy, M Richman, M Riedel, B Rodrigues, JP Rothmaier, F Rott, C Ruhe, T Rutledge, D Ruzybayev, B Ryckbosch, D Saba, SM Salameh, T Sander, HG Santander, M Sarkar, S Schatto, K Scheel, M Scheriau, F Schmidt, T Schmitz, M Schoenen, S Schoneberg, S Schonherr, L Schonwald, A Schukraft, A Schulte, L Schulz, O Seckel, D Seo, SH Sestayo, Y Seunarine, S Smith, MWE Soiron, M Soldin, D Spiczak, GM Spiering, C Stamatikos, M Stanev, T Stasik, A Stezelberger, T Stokstad, RG Stoessl, A Strahler, EA Strom, R Sullivan, GW Taavola, H Taboada, I Tamburro, A Ter-Antonyan, S Tilav, S Toale, PA Toscano, S Usner, M van Eijndhoven, N van der Drift, D Van Overloop, A van Santen, J Vehring, M Voge, M Walck, C Waldenmaier, T Wallraff, M Walter, M Wasserman, R Weaver, C Wendt, C Westerhoff, S Whitehorn, N Wiebe, K Wiebusch, CH Williams, DR Wissing, H Wolf, M Wood, TR Woschnagg, K Xu, C Xu, DL Xu, XW Yanez, JP Yodh, G Yoshida, S Zarzhitsky, P Ziemann, J Zilles, A Zoll, M AF Scott, P. Savage, C. Edsjo, J. Collaboration, IceCube Abbasi, R. Abdou, Y. Ackermann, M. Adams, J. Aguilar, J. A. Ahlers, M. Altmann, D. Andeen, K. Enberg, J. Au Ff Bai, X. Baker, M. Barwick, S. W. Baum, V. Bay, R. Beattie, K. Beatty, J. J. Bechet, S. Tjus, J. Becker Becker, K. -H. Bell, M. Benabderrahmane, M. L. BenZvi, S. Berdermann, J. Berghaus, P. Berley, D. Bernardini, E. Bertrand, D. Besson, D. Z. Bindig, D. Bissok, M. Blaufuss, E. Blumenthal, J. Boersma, D. J. Bohm, C. Bose, D. Boeser, S. Botner, O. Brayeur, L. Brown, A. M. Bruijn, R. Brunner, J. Buitink, S. Caballero-Mora, K. S. Carson, M. Casey, J. Casier, M. Chirkin, D. Christy, B. Clevermann, F. Cohen, S. Cowen, D. F. Silva, A. H. Cruz Danninger, M. Daughhetee, J. Davis, J. C. De Clercq, C. Descamps, F. Desiati, P. de Vries-Uiterweerd, G. DeYoung, T. Diaz-Velez, J. C. Dreyer, J. Dumm, J. P. Dunkman, M. Eagan, R. Eisch, J. Ellsworth, R. W. Engdegard, O. Euler, S. Evenson, P. A. Fadiran, O. Fazely, A. R. Fedynitch, A. Feintzeig, J. Feusels, T. Filimonov, K. Finley, C. Fischer-Wasels, T. Flis, S. Franckowiak, A. Franke, R. Frantzen, K. Fuchs, T. Gaisser, T. K. Gallagher, J. Gerhardt, L. Gladstone, L. Gluesenkamp, T. Goldschmidt, A. Goodman, J. A. Gora, D. Grant, D. Gross, A. Grullon, S. Gurtner, M. Ha, C. Ismail, A. Haj Hallgren, A. Halzen, F. Hanson, K. Heereman, D. Heimann, P. Heinen, D. Helbing, K. Hellauer, R. Hickford, S. Hill, G. C. Hoffman, K. D. Hoffmann, R. Homeier, A. Hoshina, K. Huelsnitz, W. Hulth, P. O. Hultqvist, K. Hussain, S. Ishihara, A. Jacobi, E. Jacobsen, J. Japaridze, G. S. Jlelati, O. Johansson, H. Kappes, A. Karg, T. Karle, A. Kiryluk, J. Kislat, F. Klaes, J. Klein, S. R. Koehne, J. -H. Kohnen, G. Kolanoski, H. Koepke, L. Kopper, C. Kopper, S. Koskinen, D. J. Kowalski, M. Krasberg, M. Kroll, G. Kunnen, J. Kurahashi, N. Kuwabara, T. Labare, M. Laihem, K. Landsman, H. Larson, M. J. Lauer, R. Lesiak-Bzdak, M. Luenemann, J. Madsen, J. Maruyama, R. Mase, K. Matis, H. S. McNally, F. Meagher, K. Merck, M. Meszaros, P. Meures, T. Miarecki, S. Middell, E. Milke, N. Miller, J. Mohrmann, L. Montaruli, T. Morse, R. Movit, S. M. Nahnhauer, R. Naumann, U. Nowicki, S. C. Nygren, D. R. Obertacke, A. Odrowski, S. Olivas, A. Olivo, M. O'Murchadha, A. Panknin, S. Paul, L. Pepper, J. A. de los Heros, C. Perez Pieloth, D. Pirk, N. Posselt, J. Price, P. B. Przybylski, G. T. Raedel, L. Rawlins, K. Redl, P. Resconi, E. Rhode, W. Ribordy, M. Richman, M. Riedel, B. Rodrigues, J. P. Rothmaier, F. Rott, C. Ruhe, T. Rutledge, D. Ruzybayev, B. Ryckbosch, D. Saba, S. M. Salameh, T. Sander, H. -G. Santander, M. Sarkar, S. Schatto, K. Scheel, M. Scheriau, F. Schmidt, T. Schmitz, M. Schoenen, S. Schoeneberg, S. Schoenherr, L. Schoenwald, A. Schukraft, A. Schulte, L. Schulz, O. Seckel, D. Seo, S. H. Sestayo, Y. Seunarine, S. Smith, M. W. E. Soiron, M. Soldin, D. Spiczak, G. M. Spiering, C. Stamatikos, M. Stanev, T. Stasik, A. Stezelberger, T. Stokstad, R. G. Stoessl, A. Strahler, E. A. Strom, R. Sullivan, G. W. Taavola, H. Taboada, I. Tamburro, A. Ter-Antonyan, S. Tilav, S. Toale, P. A. Toscano, S. Usner, M. van Eijndhoven, N. van der Drift, D. Van Overloop, A. van Santen, J. Vehring, M. Voge, M. Walck, C. Waldenmaier, T. Wallraff, M. Walter, M. Wasserman, R. Weaver, Ch. Wendt, C. Westerhoff, S. Whitehorn, N. Wiebe, K. Wiebusch, C. H. Williams, D. R. Wissing, H. Wolf, M. Wood, T. R. Woschnagg, K. Xu, C. Xu, D. L. Xu, X. W. Yanez, J. P. Yodh, G. Yoshida, S. Zarzhitsky, P. Ziemann, J. Zilles, A. Zoll, M. TI Use of event-level neutrino telescope data in global fits for theories of new physics SO JOURNAL OF COSMOLOGY AND ASTROPARTICLE PHYSICS LA English DT Article DE dark matter theory; neutrino astronomy; dark matter experiments; cosmology of theories beyond the SM ID DARK-MATTER CANDIDATES; OBSERVATIONS COSMOLOGICAL INTERPRETATION; CONSTRAINTS; SUPERSYMMETRY; LIMITS; LHC; CAPTURE; SEARCH; LIGHT AB We present a fast likelihood method for including event-level neutrino telescope data in parameter explorations of theories for new physics, and announce its public release as part of DarkSUSY 5.0.6. Our construction includes both angular and spectral information about neutrino events, as well as their total number. We also present a corresponding measure for simple model exclusion, which can be used for single models without reference to the rest of a parameter space. We perform a number of supersymmetric parameter scans with IceCube data to illustrate the utility of the method: example global fits and a signal recovery in the constrained minimal supersymmetric standard model (CMSSM), and a model exclusion exercise in a 7-parameter phenomenological version of the MSSM. The final IceCube detector con figuration will probe almost the entire focus-point region of the CMSSM, as well as a number of MSSM-7 models that will not otherwise be accessible to e. g. direct detection. Our method accurately recovers the mock signal, and provides tight constraints on model parameters and derived quantities. We show that the inclusion of spectral information significantly improves the accuracy of the recovery, providing motivation for its use in future IceCube analyses. C1 [Scott, P.] McGill Univ, Dept Phys, Montreal, PQ H3A 2T8, Canada. [Savage, C.; Edsjo, J.; Bohm, C.; Danninger, M.; Finley, C.; Flis, S.; Hulth, P. O.; Hultqvist, K.; Johansson, H.; Seo, S. H.; Walck, C.; Wolf, M.; Zoll, M.] Stockholm Univ, Oskar Klein Ctr Cosmoparticle Phys, SE-10691 Stockholm, Sweden. [Savage, C.; Edsjo, J.; Bohm, C.; Danninger, M.; Finley, C.; Flis, S.; Hulth, P. O.; Hultqvist, K.; Johansson, H.; Seo, S. H.; Walck, C.; Wolf, M.; Zoll, M.] Stockholm Univ, Dept Phys, SE-10691 Stockholm, Sweden. [Abbasi, R.; Ahlers, M.; Andeen, K.; Enberg, J. Au Ff; Baker, M.; BenZvi, S.; Chirkin, D.; Descamps, F.; Desiati, P.; Diaz-Velez, J. C.; Dumm, J. P.; Eisch, J.; Fadiran, O.; Feintzeig, J.; Gladstone, L.; Grullon, S.; Halzen, F.; Hoshina, K.; Jacobsen, J.; Karle, A.; Kopper, C.; Krasberg, M.; Kurahashi, N.; Landsman, H.; Maruyama, R.; McNally, F.; Merck, M.; Morse, R.; Riedel, B.; Rodrigues, J. P.; Santander, M.; Toscano, S.; van Santen, J.; Weaver, Ch.; Wendt, C.; Westerhoff, S.; Whitehorn, N.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Abbasi, R.; Ahlers, M.; Andeen, K.; Enberg, J. Au Ff; Baker, M.; BenZvi, S.; Chirkin, D.; Descamps, F.; Desiati, P.; Diaz-Velez, J. C.; Dumm, J. P.; Eisch, J.; Fadiran, O.; Feintzeig, J.; Gladstone, L.; Grullon, S.; Halzen, F.; Hoshina, K.; Jacobsen, J.; Karle, A.; Kopper, C.; Krasberg, M.; Kurahashi, N.; Landsman, H.; Maruyama, R.; McNally, F.; Merck, M.; Morse, R.; Riedel, B.; Rodrigues, J. P.; Santander, M.; Toscano, S.; van Santen, J.; Weaver, Ch.; Wendt, C.; Westerhoff, S.; Whitehorn, N.] Univ Wisconsin, Wisconsin IceCube Particle Astrophys Ctr, Madison, WI 53706 USA. [Abdou, Y.; Carson, M.; de Vries-Uiterweerd, G.; Feusels, T.; Ismail, A. Haj; Jlelati, O.; Ryckbosch, D.; Van Overloop, A.] Univ Ghent, Dept Phys & Astron, B-9000 Ghent, Belgium. [Ackermann, M.; Benabderrahmane, M. L.; Berdermann, J.; Berghaus, P.; Bernardini, E.; Brunner, J.; Silva, A. H. Cruz; Franke, R.; Gluesenkamp, T.; Gora, D.; Jacobi, E.; Karg, T.; Kislat, F.; Lauer, R.; Middell, E.; Mohrmann, L.; Nahnhauer, R.; Pirk, N.; Schoenwald, A.; Spiering, C.; Stoessl, A.; Walter, M.; Yanez, J. P.] DESY, D-15735 Zeuthen, Germany. [Adams, J.; Brown, A. M.; Hickford, S.] Univ Canterbury, Dept Phys & Astron, Christchurch 1, New Zealand. [Aguilar, J. A.; Montaruli, T.] Univ Geneva, Dept Phys Nucl & Corpusculaire, CH-1211 Geneva, Switzerland. [Altmann, D.; Kappes, A.; Kolanoski, H.; Waldenmaier, T.] Humboldt Univ, Inst Phys, D-12489 Berlin, Germany. [Bai, X.; Evenson, P. A.; Gaisser, T. K.; Hussain, S.; Kuwabara, T.; Ruzybayev, B.; Seckel, D.; Stanev, T.; Tamburro, A.; Tilav, S.; Xu, C.] Univ Delaware, Bartol Res Inst, Newark, DE 19716 USA. [Bai, X.; Evenson, P. A.; Gaisser, T. K.; Hussain, S.; Kuwabara, T.; Ruzybayev, B.; Seckel, D.; Stanev, T.; Tamburro, A.; Tilav, S.; Xu, C.] Univ Delaware, Dept Phys & Astron, Newark, DE 19716 USA. [Bai, X.] S Dakota Sch Mines & Technol, Dept Phys, Rapid City, SD 57701 USA. [Barwick, S. W.; Yodh, G.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. [Baum, V.; Koepke, L.; Kroll, G.; Luenemann, J.; Sander, H. -G.; Schatto, K.; Wiebe, K.] Johannes Gutenberg Univ Mainz, Inst Phys, D-55099 Mainz, Germany. [Bay, R.; Filimonov, K.; Gerhardt, L.; Ha, C.; Klein, S. R.; Miarecki, S.; Price, P. B.; Rothmaier, F.; van der Drift, D.; Woschnagg, K.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Beattie, K.; Gerhardt, L.; Goldschmidt, A.; Ha, C.; Klein, S. R.; Matis, H. S.; Miarecki, S.; Nygren, D. R.; Przybylski, G. T.; Stezelberger, T.; Stokstad, R. G.; van der Drift, D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Beatty, J. J.; Davis, J. C.; Rott, C.; Stamatikos, M.] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. [Beatty, J. J.; Davis, J. C.; Rott, C.; Stamatikos, M.] Ohio State Univ, Ctr Cosmol & Astroparticle Phys, Columbus, OH 43210 USA. [Beatty, J. J.] Ohio State Univ, Dept Astron, Columbus, OH 43210 USA. [Bechet, S.; Bertrand, D.; Hanson, K.; Heereman, D.; Meures, T.; O'Murchadha, A.] Univ Libre Bruxelles, Fac Sci, B-1050 Brussels, Belgium. [Tjus, J. Becker; Dreyer, J.; Fedynitch, A.; Olivo, M.; Saba, S. M.; Schoeneberg, S.] Ruhr Univ Bochum, Fak Phys & Astron, D-44780 Bochum, Germany. [Becker, K. -H.; Bindig, D.; Fischer-Wasels, T.; Gurtner, M.; Helbing, K.; Hoffmann, R.; Klaes, J.; Kopper, S.; Naumann, U.; Obertacke, A.; Posselt, J.; Soldin, D.] Univ Wuppertal, Dept Phys, D-42119 Wuppertal, Germany. [Bell, M.; Caballero-Mora, K. S.; Cowen, D. F.; DeYoung, T.; Dunkman, M.; Eagan, R.; Koskinen, D. J.; Meszaros, P.; Rutledge, D.; Salameh, T.; Smith, M. W. E.; Wasserman, R.] Penn State Univ, Dept Phys, University Pk, PA 16802 USA. [Berley, D.; Blaufuss, E.; Christy, B.; Ellsworth, R. W.; Goodman, J. A.; Hellauer, R.; Hoffman, K. D.; Huelsnitz, W.; Meagher, K.; Olivas, A.; Redl, P.; Richman, M.; Schmidt, T.; Sullivan, G. W.; Wissing, H.] Univ Maryland, Dept Phys, College Pk, MD 20742 USA. [Besson, D. Z.] Univ Kansas, Dept Phys & Astron, Lawrence, KS 66045 USA. [Bissok, M.; Blumenthal, J.; Boersma, D. J.; Euler, S.; Heimann, P.; Heinen, D.; Laihem, K.; Paul, L.; Raedel, L.; Scheel, M.; Schoenen, S.; Schoenherr, L.; Schukraft, A.; Soiron, M.; Vehring, M.; Wallraff, M.; Wiebusch, C. H.; Zilles, A.] Rhein Westfal TH Aachen, Inst Phys 3, D-52056 Aachen, Germany. [Bose, D.; Brayeur, L.; Buitink, S.; Casier, M.; De Clercq, C.; Kunnen, J.; Labare, M.; Miller, J.; Strahler, E. A.; van Eijndhoven, N.] Vrije Univ Brussel, Dienst ELEM, B-1050 Brussels, Belgium. [Boeser, S.; Franckowiak, A.; Homeier, A.; Kowalski, M.; Panknin, S.; Schulte, L.; Stasik, A.; Usner, M.; Voge, M.] Univ Bonn, Inst Phys, D-53115 Bonn, Germany. [Botner, O.; Engdegard, O.; Hallgren, A.; de los Heros, C. Perez; Strom, R.; Taavola, H.] Uppsala Univ, Dept Phys & Astron, S-75120 Uppsala, Sweden. [Bruijn, R.; Cohen, S.; Ribordy, M.] Ecole Polytech Fed Lausanne, High Energy Phys Lab, CH-1015 Lausanne, Switzerland. [Casey, J.; Daughhetee, J.; Taboada, I.] Georgia Inst Technol, Sch Phys, Atlanta, GA 30332 USA. [Casey, J.; Daughhetee, J.; Taboada, I.] Georgia Inst Technol, Ctr Relativist Astrophys, Atlanta, GA 30332 USA. [Clevermann, F.; Frantzen, K.; Fuchs, T.; Koehne, J. -H.; Milke, N.; Pieloth, D.; Rhode, W.; Ruhe, T.; Scheriau, F.; Schmitz, M.; Ziemann, J.] TU Dortmund Univ, Dept Phys, D-44221 Dortmund, Germany. [Cowen, D. F.; Meszaros, P.; Movit, S. M.] Penn State Univ, Dept Astron & Astrophys, University Pk, PA 16802 USA. [Fazely, A. R.; Ter-Antonyan, S.; Xu, X. W.] Southern Univ, Dept Phys, Baton Rouge, LA 70813 USA. [Gallagher, J.] Univ Wisconsin, Dept Astron, Madison, WI 53706 USA. [Grant, D.; Nowicki, S. C.; Wood, T. R.] Univ Alberta, Dept Phys, Edmonton, AB T6G 2G7, Canada. [Gross, A.; Odrowski, S.; Resconi, E.; Schulz, O.; Sestayo, Y.] Tech Univ Munich, D-85748 Garching, Germany. [Hill, G. C.] Univ Adelaide, Sch Chem & Phys, Adelaide, SA 5005, Australia. [Huelsnitz, W.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Ishihara, A.; Mase, K.; Yoshida, S.] Chiba Univ, Dept Phys, Chiba 2638522, Japan. [Japaridze, G. S.] Clark Atlanta Univ, CTSPS, Atlanta, GA 30314 USA. [Kiryluk, J.; Lesiak-Bzdak, M.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Kohnen, G.] Univ Mons, B-7000 Mons, Belgium. [Larson, M. J.; Pepper, J. A.; Toale, P. A.; Williams, D. R.; Xu, D. L.; Zarzhitsky, P.] Univ Alabama, Dept Phys & Astron, Tuscaloosa, AL 35487 USA. [Madsen, J.; Spiczak, G. M.] Univ Wisconsin, Dept Phys, River Falls, WI 54022 USA. [Montaruli, T.] Univ Bari, Dipartmento Fis, Sez INFN, I-70126 Bari, Italy. [Rawlins, K.] Univ Alaska Anchorage, Dept Phys & Astron, Anchorage, AK 99508 USA. [Sarkar, S.] Univ Oxford, Dept Phys, Oxford OX1 3NP, England. [Seunarine, S.] Univ W Indies, Dept Phys, BB-11000 Bridgetown, Barbados. [Stamatikos, M.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. RP Scott, P (reprint author), McGill Univ, Dept Phys, 3600 Rue Univ, Montreal, PQ H3A 2T8, Canada. EM patscott@physics.mcgill.ca; savage@fysik.su.se; danning@fysik.su.se RI Wiebusch, Christopher/G-6490-2012; Koskinen, David/G-3236-2014; Brunner, Juergen/G-3540-2015; Maruyama, Reina/A-1064-2013; Sarkar, Subir/G-5978-2011; Beatty, James/D-9310-2011; Tamburro, Alessio/A-5703-2013; Botner, Olga/A-9110-2013; Hallgren, Allan/A-8963-2013; Tjus, Julia/G-8145-2012 OI Aguilar Sanchez, Juan Antonio/0000-0003-2252-9514; Wiebusch, Christopher/0000-0002-6418-3008; Koskinen, David/0000-0002-0514-5917; Brunner, Juergen/0000-0002-5052-7236; Maruyama, Reina/0000-0003-2794-512X; Sarkar, Subir/0000-0002-3542-858X; Beatty, James/0000-0003-0481-4952; Rott, Carsten/0000-0002-6958-6033; Ter-Antonyan, Samvel/0000-0002-5788-1369; Schukraft, Anne/0000-0002-9112-5479; FU Lorne Trottier Chair in Astrophysics; Canadian Institute for Particle Physics Theory Fellowship; Swedish Research Council [621-2010-3705, 621-2010-3301]; U.S. National Science Foundation - Office of Polar Programs; U.S. National Science Foundation - Physics Division; University of Wisconsin Alumni Research Foundation; Grid Laboratory Of Wisconsin (GLOW); U.S. Department of Energy; National Energy Research Scientific Computing Center; Louisiana Optical Network Initiative (LONI); National Science and Engineering Research Council of Canada; Swedish Research Council; Swedish Polar Research Secretariat; Swedish National Infrastructure for Computing (SNIC); Knut and Alice Wallenberg Foundation, Sweden; German Ministry for Education and Research (BMBF); Deutsche Forschungsgemeinschaft (DFG); Research Department of Plasmas with Complex Interactions (Bochum), Germany; Fund for Scientific Research (FNRS-FWO); FWO Odysseus programme; Flanders Institute to encourage scientific and technological research in industry (IWT); Belgian Federal Science Policy - Office (Belspo); University of Oxford, United Kingdom; Marsden Fund, New Zealand; Australian Research Council; Japan Society for Promotion of Science (JSPS); Swiss National Science Foundation (SNSF), Switzerland FX We are grateful to Hamish Silverwood for helpful comments and discussions. P. S. is supported by the Lorne Trottier Chair in Astrophysics and a Canadian Institute for Particle Physics Theory Fellowship. M. D. and K. H. acknowledge support from the Swedish Research Council (Contract No. 621-2010-3705), as does J.E. (Contract No. 621-2010-3301).; We acknowledge the support from the following agencies: U.S. National Science Foundation - Office of Polar Programs, U.S. National Science Foundation - Physics Division, University of Wisconsin Alumni Research Foundation, the Grid Laboratory Of Wisconsin (GLOW) grid infrastructure at the University of Wisconsin {Madison, the Open Science Grid (OSG) grid infrastructure; U.S. Department of Energy, and National Energy Research Scientific Computing Center, the Louisiana Optical Network Initiative (LONI) grid computing resources; National Science and Engineering Research Council of Canada; Swedish Research Council, Swedish Polar Research Secretariat, Swedish National Infrastructure for Computing (SNIC), and Knut and Alice Wallenberg Foundation, Sweden; German Ministry for Education and Research (BMBF), Deutsche Forschungsgemeinschaft (DFG), Research Department of Plasmas with Complex Interactions (Bochum), Germany; Fund for Scientific Research (FNRS-FWO), FWO Odysseus programme, Flanders Institute to encourage scientific and technological research in industry (IWT), Belgian Federal Science Policy - Office (Belspo); University of Oxford, United Kingdom; Marsden Fund, New Zealand; Australian Research Council; Japan Society for Promotion of Science (JSPS); the Swiss National Science Foundation (SNSF), Switzerland. NR 102 TC 18 Z9 18 U1 0 U2 8 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1475-7516 J9 J COSMOL ASTROPART P JI J. Cosmol. Astropart. Phys. PD NOV PY 2012 IS 11 AR 057 DI 10.1088/1475-7516/2012/11/057 PG 33 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 053IA UT WOS:000312263500040 ER PT J AU Aad, G Abajyan, T Abbott, B Abdallah, J Khalek, SA Abdelalim, AA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Acerbi, E Acharya, BS Adamczyk, L Adams, DL Addy, TN Adelman, J Adomeit, S Adragna, P Adye, T Aefsky, S Aguilar-Saavedra, JA Agustoni, M Aharrouche, M Ahlen, SP Ahles, F Ahmad, A Ahsan, M Aielli, G Akdogan, T Akesson, TPA Akimoto, G Akimov, AV Alam, MS Alam, MA Albert, J Albrand, S Aleksa, M Aleksandrov, IN Alessandria, F Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Aliev, M Alimonti, G Alison, J Allbrooke, BMM Allport, PP Allwood-Spiers, SE Almond, J Aloisio, A Alon, R Alonso, A Alonso, F Gonzalez, BA Alviggi, MG Amako, K Amelung, C Ammosov, VV Amorim, A Amram, N Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Anduaga, XS Anger, P Angerami, A Anghinolfi, F Anisenkov, A Anjos, N Annovi, A Antonaki, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Aoun, S Bella, LA Apolle, R Arabidze, G Aracena, I Arai, Y Arce, ATH Arfaoui, S Arguin, JF Arik, E Arik, M Armbruster, AJ Arnaez, O Arnal, V Arnault, C Artamonov, A Artoni, G Arutinov, D Asai, S Asfandiyarov, R Ask, S Asman, B Asquith, L Assamagan, K Astbury, A Atkinson, M Aubert, B Auge, E Augsten, K Aurousseau, M Avolio, G Avramidou, R Axen, D Azuelos, G Azuma, Y Baak, MA Baccaglioni, G Bacci, C Bach, AM Bachacou, H Bachas, K Backes, M Backhaus, M Badescu, E Bagnaia, P Bahinipati, S Bai, Y Bailey, DC Bain, T Baines, JT Baker, OK Baker, MD Baker, S Banas, E Banerjee, P Banerjee, S Banfi, D Bangert, A Bansal, V Bansil, HS Barak, L Baranov, SP Galtieri, AB Barber, T Barberio, EL Barberis, D Barbero, M Bardin, DY Barillari, T Barisonzi, M Barklow, T Barlow, N Barnett, BM Barnett, RM Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Barrillon, P Bartoldus, R Barton, AE Bartsch, V Basye, A Bates, RL Batkova, L Batley, JR Battaglia, A Battistin, M Bauer, F Bawa, HS Beale, S Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, AK Becker, S Beckingham, M Becks, KH Beddall, AJ Beddall, A Bedikian, S Bednyakov, VA Bee, CP Beemster, LJ Begel, M Harpaz, SB Beimforde, M Belanger-Champagne, C Bell, PJ Bell, WH Bella, G Bellagamba, L Bellina, F Bellomo, M Belloni, A Beloborodova, O Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Benoit, M Bensinger, JR Benslama, K Bentvelsen, S Berge, D Kuutmann, EB Berger, N Berghaus, F Berglund, E Beringer, J Bernat, P Bernhard, R Bernius, C Berry, T Bertella, C Bertin, A Bertolucci, F Besana, MI Besjes, GJ Besson, N Bethke, S Bhimji, W Bianchi, RM Bianco, M Biebel, O Bieniek, SP Bierwagen, K Biesiada, J Biglietti, M Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Biscarat, C 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CA ATLAS Collaboration TI Measurements of the pseudorapidity dependence of the total transverse energy in proton-proton collisions at root s=7 TeV with ATLAS SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering ID PARTON DISTRIBUTIONS; CROSS-SECTION; QCD ANALYSIS; CALORIMETER; REGION; LHC AB This paper describes measurements of the sum of the transverse energy of particles as a function of particle pseudorapidity, eta, in proton-proton collisions at a centre-of-mass energy, root s = 7 TeV using the ATLAS detector at the Large Hadron Collider. The measurements are performed in the region \eta\ < 4.8 for two event classes: those requiring the presence of particles with a low transverse momentum and those requiring particles with a significant transverse momentum. In the second dataset measurements are made in the region transverse to the hard scatter. 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L.; Assamagan, K.; Baker, M. D.; Begel, M.; Bernius, C.; Chen, H.; Chernyatin, V.; Debbe, R.; Dhullipudi, R.; Ernst, M.; Gadfort, T.; Gibbard, B.; Gordon, H. A.; Greenwood, Z. D.; Klimentov, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Majewski, S.; Metcalfe, J.; Nevski, P.; Okawa, H.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Park, W.; Pleier, M. -A.; Poblaguev, A.; Polychronakos, V.; Pravahan, R.; Protopopescu, S.; Purohit, M.; Rahm, D.; Rajagopalan, S.; Redlinger, G.; Sawyer, L.; Sircar, A.; Snyder, S.; Steinberg, P.; Stumer, I.; Takai, H.; Tamsett, M. C.; Triplett, N.; Undrus, A.; Wenaus, T.; Ye, S.; Yu, D.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Badescu, E.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Cuciuc, C. -M.; Dinut, F.; Dita, P.; Dita, S.; Micu, L.; Olariu, A.; Pantea, D.; Popeneciu, G. A.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Darlea, G. L.] Univ Politehn Bucuresti, Bucharest, Romania. W Univ Timisoara, Timisoara, Romania. [Gonzalez Silva, M. L.; Garzon, G. Otero Y.; Piegaia, R.; Romeo, G.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Ask, S.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Buttinger, W.; Carter, J. R.; Chapman, J. D.; Cowden, C.; French, S. T.; Frost, J. A.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Moeller, V.; Parker, M. A.; Robinson, D.; Sandoval, T.; Thomson, M.; Ward, C. P.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Gillberg, D.; Koffas, T.; Liu, C.; Marchand, J. F.; McCarthy, T. G.; Oakham, F. G.; Randrianarivony, K.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Anastopoulos, C.; Anghinolfi, F.; Baak, M. A.; Bachas, K.; Banfi, D.; Battistin, M.; Bellina, F.; Bellomo, M.; Beltramello, O.; Berge, D.; Bianchi, R. M.; Blanchot, G.; Bogaerts, J. A.; Boyd, J.; Bremer, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Catmore, J. R.; Cattai, A.; Cerri, A.; Barajas, C. A. Chavez; Childers, J. T.; Chromek-Burckhart, D.; Cote, D.; Danielsson, H. O.; Dell'Acqua, A.; Di Girolamo, A.; Di Girolamo, B.; Di Micco, B.; Dittus, F.; Dobinson, R.; Dobos, D.; Dobson, E.; Dopke, J.; Dudarev, A.; Duehrssen, M.; Dunford, M.; Dydak, F.; Ellis, N.; Elsing, M.; Fabre, C.; Farthouat, P.; Fassnacht, P.; Francis, D.; Franz, S.; Froeschl, R.; Froidevaux, D.; Torregrosa, E. Fullana; Gabaldon, C.; Garelli, N.; Garonne, V.; Gianotti, F.; Gibson, S. M.; Godlewski, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Haas, S.; Hahn, F.; Haider, S.; Hauschild, M.; Hawkings, R. J.; Heller, M.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Huhtinen, M.; Inigo-Golfin, J.; Jaekel, M. R.; Jansen, H.; Jenni, P.; Joram, C.; Jungst, R. M.; Kaneda, M.; Kaplon, J.; Kerschen, N.; Klioutchnikova, T.; Koeneke, K.; Lamanna, M.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Malaescu, B.; Malyukov, S.; Mapelli, A.; Mapelli, L.; Marshall, Z.; Martin, B.; Messina, A.; Meyer, T. C.; Michal, S.; Morley, A. K.; Mornacchi, G.; Muenstermann, D.; Nairz, A. M.; Nakahama, Y.; Negri, G.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Ohm, C. C.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Petersen, J.; Piacquadio, G.; Pommes, K.; Poppleton, A.; Bueso, X. Portell; Poulard, G.; Prasad, S.; Raymond, M.; Rembser, C.; Dos Santos, D. Roda; Roe, S.; Salek, D.; Salzburger, A.; Savu, D. O.; Schlenker, S.; Schott, M.; Sfyrla, A.; Spigo, G.; Spiwoks, R.; Stewart, G. A.; Teischinger, F. A.; Ten Kate, H.; Torchiani, I.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van der Ster, D.; van Eldik, N.; Vandelli, W.; Veness, R.; Vinek, E.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Winklmeier, F.; Wotschack, J.; Byszewski, M.; Zajacova, Z.; Zwalinski, L.] CERN, Geneva, Switzerland. [Anderson, K. J.; Boveia, A.; Canelli, F.; Choudalakis, G.; Costin, T.; Fiascaris, M.; Gardner, R. W.; Jen-La Plante, I.; Kapliy, A.; Melachrinos, C.; Merritt, F. S.; Meyer, C.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Shochet, M. J.; Tompkins, L.; Tuggle, J. M.; Vukotic, I.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Diaz, M. A.; Olivares Pino, S. A.; Quinonez, F.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Carquin, E.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Jin, S.; Lu, F.; Ouyang, Q.; Ruan, X.; Shan, L. Y.; Yao, L.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Han, L.; Jiang, Y.; Li, S.; Liu, M.; Liu, Y.; Peng, H.; Wang, H.; Wu, Y.; Xu, C.; Zhang, D.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Feng, C.; Ge, P.; He, M.; Miao, J.; Zhan, Z.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Toro, R. Camacho; Cinca, D.; Donini, J.; Febbraro, R.; Ghodbane, N.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Vazeille, F.] Clermont Univ, Phys Corpusculaire Lab, Aubiere, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Toro, R. Camacho; Cinca, D.; Donini, J.; Febbraro, R.; Ghodbane, N.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Vazeille, F.] Univ Clermont Ferrand, Aubiere, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Toro, R. Camacho; Cinca, D.; Donini, J.; Febbraro, R.; Ghodbane, N.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Vazeille, F.] IN2P3, CNRS, Aubiere, France. [Andeen, T.; Angerami, A.; Brooijmans, G.; Chen, Y.; Dodd, J.; Grau, N.; Guo, J.; Hu, D.; Hughes, E. W.; Nikiforou, N.; Parsons, J. A.; Penson, A.; Perez, K.; Reale, V. Perez; Scherzer, M. I.; Spousta, M.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Williams, E.; Willis, W.; Wulf, E.; Zivkovic, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Boelaert, N.; Dam, M.; Gregersen, K.; Hansen, J. R.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Heisterkamp, S.; Jakobsen, S.; Loevschall-Jensen, A. E.; Jez, P.; Joergensen, M. D.; Kadlecik, P.; Klinkby, E. B.; Lundquist, J.; Mackeprang, R.; Mehlhase, S.; Petersen, T. C.; Simonyan, M.; Thomsen, L. A.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; Fazio, S.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Morello, G.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Grp Collegato Cosenza, Arcavacata Di Rende, Italy. [Capua, M.; Crosetti, G.; Fazio, S.; La Rotonda, L.; Lavorini, V.; Mastroberardino, A.; Morello, G.; Policicchio, A.; Salvatore, D.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Banas, E.; Blocki, J.; de Renstrom, P. A. Bruckman; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Malecki, P.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Turala, M.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.; Zemla, A.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Yagci, K. Dindar; Firan, A.; Hadavand, H. K.; Hoffman, J.; Ishmukhametov, R.; Joffe, D.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Rios, R. R.; Sekula, S. J.; Stroynowski, R.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Ahsan, M.; Izen, J. M.; Lou, X.; Reeves, K.; Wong, W. C. .] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Kuutmann, E. Bergeaas; Dassoulas, J. A.; Dietrich, J.; Ehrenfeld, W.; Ferrara, V.; Fischer, G.; Friedrich, C.; Glazov, A.; Goebel, M.; Fajardo, L. S. Gomez; Firmino Da Costa, J. Goncalves Pinto; Gosdzik, B.; Grahn, K. J.; Gregor, I. M.; Hiller, K. H.; Huettmann, A.; Husemann, U.; Belenguer, M. Jimenez; Johnert, S.; Karnevskiy, M.; Katzy, J.; Kono, T.; Kuhl, T.; Lange, C.; Lobodzinska, E.; Ludwig, D.; Medinnis, M.; Moenig, K.; Naumann, T.; Cavalcanti, T. Perez; Petschu, D.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Stanescu-Bellu, M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Zhu, H.] DESY, D-2000 Hamburg, Germany. [Kuutmann, E. Bergeaas; Dassoulas, J. A.; Dietrich, J.; Ehrenfeld, W.; Ferrara, V.; Fischer, G.; Friedrich, C.; Glazov, A.; Goebel, M.; Fajardo, L. S. Gomez; Firmino Da Costa, J. Goncalves Pinto; Gosdzik, B.; Grahn, K. J.; Gregor, I. M.; Hiller, K. H.; Huettmann, A.; Husemann, U.; Belenguer, M. Jimenez; Johnert, S.; Karnevskiy, M.; Katzy, J.; Kono, T.; Kuhl, T.; Lange, C.; Lobodzinska, E.; Ludwig, D.; Medinnis, M.; Moenig, K.; Naumann, T.; Cavalcanti, T. Perez; Petschu, D.; Piec, S. M.; Radescu, V.; Rubinskiy, I.; Sedov, G.; Stanescu-Bellu, M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Vankov, P.; Viti, M.; Wasicki, C.; Wildt, M. A.; Zhu, H.] DESY, Zeuthen, Germany. [Bunse, M.; Esch, H.; Goessling, C.; Hirsch, F.; Jung, C. A.; Klingenberg, R.; Reisinger, I.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Czodrowski, P.; Friedrich, F.; Goepfert, T.; Kobel, M.; Leonhardt, K.; Ludwig, A.; Mader, W. F.; Morgenstern, M.; Prudent, X.; Rudolph, C.; Schnoor, U.; Schwierz, R.; Seifert, F.; Steinbach, P.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Ko, B. R.; Kotwal, A.; Oh, S. H.; Wang, C.; Yamaoka, J.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Buckley, A. G.; Clark, P. J.; Debenedetti, C.; Harrington, R. D.; Martin, V. J.; O'Brien, B. J.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Cerutti, F.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Sansoni, A.; Testa, M.; Vilucchi, E.; Volpi, G.] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Abdelalim, A. A.; Alexandre, G.; Backes, M.; Barone, G.; Bell, P. J.; Bell, W. H.; Noccioli, E. Benhar; Blondel, A.; Bucci, F.; Clark, A.; Dao, V.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Iacobucci, G.; La Rosa, A.; Lister, A.; Latour, B. Martin Dit; Mermod, P.; Herrera, C. Mora; Nektarijevic, S.; Nessi, M.; Nikolics, K.; Pasztor, G.; Picazio, A.; Pohl, M.; Rosbach, K.; Rosselet, L.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Beccherle, R.; Caso, C.; Dameri, M.; Darbo, G.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Barberis, D.; Caso, C.; Dameri, M.; Parodi, A. Ferretto; Gagliardi, G.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Chikovani, L.; Tskhadadze, E. G.] Tbilisi State Univ, E Andronikashvili Inst Phys, GE-380086 Tbilisi, Rep of Georgia. [Djobava, T.; Khubua, J.; Mchedlidze, G.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Stenzel, H.] Univ Giessen, Inst Phys 2, D-6300 Giessen, Germany. [Allwood-Spiers, S. E.; Bates, R. L.; Britton, D.; Bussey, P.; Buttar, C. M.; Collins-Tooth, C.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Edwards, N. C.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Kar, D.; Kenyon, M.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Robson, A.; Saxon, D. H.; Smith, K. M.; St Denis, R. D.; Steele, G.; Thompson, A. S.; Wraight, K.; Wright, M.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Bierwagen, K.; Blumenschein, U.; Brandt, O.; Erdmann, J.; Evangelakou, D.; George, M.; Grosse-Knetter, J.; Guindon, S.; Haller, J.; Hamer, M.; Henrichs, A.; Hensel, C.; Keil, M.; Knue, A.; Kohn, F.; Krieger, N.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Mann, A.; Meyer, J.; Morel, J.; Pashapour, S.; Quadt, A.; Roe, A.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Uhrmacher, M.; Schroeder, T. Vazquez; Weber, P.; Weingarten, J.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Stark, J.; Sun, X.; Trocme, B.; Wang, J.; Weydert, C.] Univ Grenoble 1, Lab Phys Subatom & Cosmol, Grenoble, France. [Albrand, S.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Stark, J.; Sun, X.; Trocme, B.; Wang, J.; Weydert, C.] IN2P3, CNRS, Grenoble, France. [Albrand, S.; Buat, Q.; Clement, B.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delemontex, T.; Delsart, P. A.; Genest, M. H.; Hostachy, J-Y.; Laisne, E.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Stark, J.; Sun, X.; Trocme, B.; Wang, J.; Weydert, C.] Inst Natl Polytech Grenoble, F-38031 Grenoble, France. [Addy, T. N.; Harvey, A.; McFarlane, K. W.; Shin, T.; Vassilakopoulos, V. I.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Belloni, A.; Catastini, P.; Conti, G.; Huth, J.; Jeanty, L.; Kagan, M.; Mateos, D. Lopez; Outschoorn, V. Martinez; Mercurio, K. M.; Mills, C.; Morii, M.; Skottowe, H. P.; Smith, B. C.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Anders, G.; Andrei, V.; Davygora, Y.; Dietzsch, T. A.; Geweniger, C.; Hanke, P.; Henke, M.; Khomich, A.; Kluge, E. -E.; Lang, V. S.; Lendermann, V.; Lepold, F.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, D-6900 Heidelberg, Germany. [Kugel, A.; Maenner, R.; Schroer, N.] Heidelberg Univ, ZITI Inst Tech Informat, D-6800 Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Cwetanski, P.; Evans, H.; Gagnon, P.; Jain, V.; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Price, D.; Whittington, D.; Yang, Y.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Beloborodova, O.; Epp, B.; Jussel, P.; Kneringer, E.; Kuhn, D.; Lukas, W.; Rudolph, G.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Limper, M.; Mallik, U.; Pylypchenko, Y.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Rosenberg, E. I.; Ruiz-Martinez, A.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Aleksandrov, I. N.; Bardin, D. Y.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Grigalashvili, N.; Huseynov, N.; Kalinovskaya, L. V.; Kazarinov, M. Y.; Kekelidze, G. D.; Kharchenko, D.; Khramov, E.; Kolesnikov, V.; Kotov, V. M.; Kruchonak, U.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Pozdnyakov, V.; Rumyantsev, L.; Rusakovich, N. A.; Sadykov, R.; Shiyakova, M.; Sisakyan, A. N.; Topilin, N. D.; Vinogradov, V. B.; Zhemchugov, A.; Zimin, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Arai, Y.; Doi, Y.; Haruyama, T.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Makida, Y.; Manabe, A.; Mitsui, S.; Nagano, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Hayakawa, T.; King, M.; Kishimoto, T.; Kitamura, T.; Kurashige, H.; Matsushita, T.; Ochi, A.; Suzuki, Y.; Takeda, H.; Tani, K.; Watanabe, I.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Sasao, N.; Sumida, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Tripiana, M. F.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Davidson, R.; de Mora, L.; Dearnaley, W. J.; Fox, H.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Konoplich, R.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Bianco, M.; Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Bianco, M.; Cataldi, G.; Chiodini, G.; Gorini, E.; Grancagnolo, F.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Greenshaw, T.; Gwilliam, C. B.; Hayward, H. S.; Jackson, J. N.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kluge, T.; Kretzschmar, J.; Laycock, P.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Sellers, G.; Vossebeld, J. H.; Waller, P.; Wrona, B.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Dolenc, I.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Dolenc, I.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Tykhonov, A.] Univ Ljubljana, Ljubljana, Slovenia. [Adragna, P.; Bona, M.; Carter, A. A.; Cerrito, L.; Eisenhandler, E.; Ellis, K.; Goddard, J. R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Poll, J.; Rizvi, E.; Salamanna, G.; Castanheira, M. Teixeira Dias; Wiglesworth, C.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Alam, M. A.; Berry, T.; Boisvert, V.; Brooks, T.; Cantrill, R.; Cowan, G.; Duguid, L.; Edwards, C. A.; George, S.; Goncalo, R.; Hayden, D.; Pastore, Fr.; Rose, M.; Spano, F.; Strong, J. A.; Teixeira-Dias, P.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Baker, S.; Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Chislett, R. T.; Christidi, I. A.; Cooper, B. D.; Davison, A. R.; Dobson, E.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Lambourne, L.; Monk, J.; Nash, M.; Nurse, E.; Prabhu, R.; Sherwood, P.; Simmons, B.; Taylor, C.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Cavalleri, P.; Chareyre, E.; Davignon, O.; De Cecco, S.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph; Theveneaux-Pelzer, T.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Cavalleri, P.; Chareyre, E.; Davignon, O.; De Cecco, S.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph; Theveneaux-Pelzer, T.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Bordoni, S.; Calderini, G.; Cavalleri, P.; Chareyre, E.; Davignon, O.; De Cecco, S.; Derue, F.; Krasny, M. W.; Kuna, M.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Ridel, M.; Roos, L.; Schwemling, Ph; Theveneaux-Pelzer, T.; Torres, H.; Trincaz-Duvoid, S.; Vannucci, F.] IN2P3, CNRS, Paris, France. [Akesson, T. P. A.; Alonso, A.; Bocchetta, S. S.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Jarlskog, G.; Lundberg, B.; Lytken, E.; Meirose, B.; Mjoernmark, J. U.; Smirnova, O.] Lund Univ, Inst Fys, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Labarga, L.; Lagouri, T.; Merino, J. Llorente; March, L.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Aharrouche, M.; Arnaez, O.; Blum, W.; Buescher, V.; Caputo, R.; Eckweiler, S.; Edmonds, K.; Ellinghaus, F.; Ertel, E.; Fiedler, F.; Fleckner, J.; Goeringer, C.; Handel, C.; Hohlfeld, M.; Hsu, P. J.; Ji, W.; Kawamura, G.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lungwitz, M.; Maettig, S.; Masetti, L.; Meyer, C.; Moreno, D.; Mueller, T.; Neusiedl, A.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schroeder, C.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.] Johannes Gutenberg Univ Mainz, Inst Phys, D-6500 Mainz, Germany. [Almond, J.; Borri, M.; Brown, G.; Chavda, V.; Cox, B. E.; Da Via, C.; Duerdoth, I. P.; Forti, A.; Howarth, J.; Ibbotson, M.; Joshi, K. D.; Klinger, J. A.; Lane, J. L.; Loebinger, F. K.; Marx, M.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Pilkington, A. D.; Robinson, J. E. M.; Schwanenberger, C.; Snow, S. W.; Watts, S.; Woudstra, M. J.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aoun, S.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Li, S.; Maurer, J.; Monnier, E.; Odier, J.; Pralavorio, P.; Rozanov, A.; Talby, M.; Tannoury, N.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aoun, S.; Bee, C. P.; Bertella, C.; Bousson, N.; Clemens, J. C.; Coadou, Y.; Djama, F.; Etienne, F.; Feligioni, L.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Li, S.; Maurer, J.; Monnier, E.; Odier, J.; Pralavorio, P.; Rozanov, A.; Talby, M.; Tannoury, N.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] IN2P3, CNRS, Marseille, France. [Brau, B.; Colon, G.; Dallapiccola, C.; Meade, A.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Varol, T.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Caron, B.; Chapleau, B.; Cheatham, S.; Corriveau, F.; Dobbs, M.; Dufour, M-A.; Guler, H.; Klemetti, M.; Mc Donald, J.; Robertson, S. H.; Rios, C. Santamarina; Schram, M.; Stockton, M. C.; Vachon, B.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Davidson, N.; Diglio, S.; Jennens, D.; Kubota, T.; Limosani, A.; Moorhead, G. F.; Hanninger, G. Nunes; Phan, A.; Shao, Q. T.; Soni, N.; Taylor, G. N.; Thong, W. M.; Volpi, M.; White, M. J.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Armbruster, A. J.; Borroni, S.; Chapman, J. W.; Cirilli, M.; Dai, T.; Diehl, E. B.; Ferretti, C.; Goldfarb, S.; Harper, D.; Levin, D.; Li, X.; Liu, H.; Liu, J. B.; Liu, L.; Mc Kee, S. P.; Neal, H. A.; Panikashvili, N.; Purdham, J.; Qian, J.; Scheirich, D.; Thun, R. P.; Walch, S.; Wilson, A.; Wooden, G.; Wu, Y.; Yang, H.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Fedorko, W.; Hauser, R.; Heim, S.; Holzbauer, J. L.; Huston, J.; Koll, J.; Linnemann, J. T.; Mangeard, P. S.; Martin, B.; Miller, R. J.; Pope, B. G.; Schwienhorst, R.; Stelzer, H. J.; Tollefson, K.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Acerbi, E.; Andreazza, A.; Besana, M. I.; Carminati, L.; Consonni, S. M.; Fanti, M.; Favareto, A.; Meloni, F.; Perini, L.; Pizio, C.; Ragusa, F.; Rivoltella, G.; Simoniello, R.; Turra, R.; Vegni, G.] Univ Milan, Dipartimento Fis, Milan, Italy. [Acerbi, E.; Alessandria, F.; Alimonti, G.; Andreazza, A.; Baccaglioni, G.; Besana, M. I.; Broggi, F.; Carminati, L.; Cavalli, D.; Citterio, M.; Consonni, S. M.; Costa, G.; Fanti, M.; Favareto, A.; Giugni, D.; Koletsou, I.; Lari, T.; Mandelli, L.; Mazzanti, M.; Meloni, F.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Rivoltella, G.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Vegni, G.; Volpini, G.] Ist Nazl Fis Nucl, Sez Milano, I-20133 Milan, Italy. [Bogouch, A.; Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Satsounkevitch, I.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus. [Yanush, S.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Azuelos, G.; Banerjee, P.; Bouchami, J.; Davies, M.; Giunta, M.; Leroy, C.; Martin, J. P.; Mehdiyev, R.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Baranov, S. P.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.] Russian Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Khodinov, A.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu; Smirnov, Y.; Soldatov, E. Yu; Timoshenko, S.] Moscow Engn & Phys Inst MEPhI, Moscow, Russia. [Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Rud, V. I.; Sivoklokov, S. Yu; Smirnova, L. N.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Beale, S.; Becker, S.; Biebel, O.; Calfayan, P.; De Graat, J.; Duckeck, G.; Ebke, J.; Elmsheuser, J.; Engl, A.; Galea, C.; Heller, C.; Hertenberger, R.; Kummer, C.; Legger, F.; Lichtnecker, M.; Lorenz, J.; Mameghani, R.; Mueller, T. A.; Nunnemann, T.; Oakes, L. B.; Rauscher, F.; Reznicek, P.; Sanders, M. P.; Schaile, D.; Schieck, J.; Serfon, C.; Staude, A.; Vladoiu, D.; Walker, R.; Will, J. Z.; Zhuang, X.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Beimforde, M.; Bethke, S.; Bittner, B.; Bronner, J.; Capriotti, D.; Cortiana, G.; Dubbert, J.; Flowerdew, M. J.; Giovannini, P.; Jantsch, A.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kotov, S.; Kroha, H.; Macchiolo, A.; Manfredini, A.; Menke, S.; Moser, H. G.; Nagel, M.; Nisius, R.; Oberlack, H.; Pahl, C.; Pospelov, G. E.; Potrap, I. N.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph; Seuster, R.; Stern, S.; Stonjek, S.; Vanadia, M.; von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.; Zhuravlov, V.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Shimizu, S.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Aoki, M.; Hasegawa, S.; Morvaj, L.; Ohshima, T.; Shimizu, S.; Takahashi, Y.; Tomoto, M.; Wakabayashi, J.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Capasso, L.; Carlino, G.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; della Volpe, D.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Musto, E.; Patricelli, S.; Sanchez, A.; Sekhniaidze, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Capasso, L.; Chiefari, G.; della Volpe, D.; Giordano, R.; Merola, L.; Musto, E.; Patricelli, S.; Sanchez, A.] Univ Naples Federico II, Dipartimento Sci Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Chelstowska, M. A.; De Groot, N.; Filthaut, F.; Klok, P. F.; Koenig, A. C.; Koetsveld, F.; Raas, M.; Salvucci, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Colijn, A. P.; De Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Doxiadis, A. D.; Ferrari, P.; Garitaonandia, H.; Geerts, D. A. A.; Gosselink, M.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kayl, M. S.; Klous, S.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Luijckx, G.; Massaro, G.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Pani, P.; Rijpstra, M.; Ruckstuhl, N.; Ta, D.; Tsiakiris, M.; Turlay, E.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuwl, R.; van der Poel, E.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Beemster, L. J.; Bentvelsen, S.; Berglund, E.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Colijn, A. P.; De Jong, P.; De Nooij, L.; Deluca, C.; Deviveiros, P. O.; Doxiadis, A. D.; Ferrari, P.; Garitaonandia, H.; Geerts, D. A. A.; Gosselink, M.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kayl, M. S.; Klous, S.; Kluit, P.; Koffeman, E.; Lee, H.; Lenz, T.; Linde, F.; Luijckx, G.; Massaro, G.; Mechnich, J.; Mussche, I.; Ottersbach, J. P.; Pani, P.; Rijpstra, M.; Ruckstuhl, N.; Ta, D.; Tsiakiris, M.; Turlay, E.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van der Leeuwl, R.; van der Poel, E.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.] Univ Amsterdam, Amsterdam, Netherlands. [Calkins, R.; Chakraborty, D.; Cole, S.; de Lima, J. G. Rocha; Suhr, C.; Yurkewicz, A.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL USA. [Anisenkov, A.; Beloborodova, O.; Bobrovnikov, V. B.; Bogdanchikov, A.; Kazanin, V. A.; Kolachev, G. M.; Korol, A.; Malyshev, V.; Maslennikov, A. L.; Orlov, I.; Peleganchuk, S. V.; Schamov, A. G.; Skovpen, K.; Soukharev, A.; Talyshev, A.; Tikhonov, Y. A.; Zaytsev, A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Budick, B.; Casadei, D.; Cranmer, K.; van Huysduynen, L. Hooft; Kaplan, B.; Konoplich, R.; Krasznahorkay, A.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.; Prokofiev, K.; Shibata, A.; Zhao, L.] NYU, Dept Phys, New York, NY 10003 USA. [Fisher, M. J.; Gan, K. K.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Rahimi, A. M.; Strang, M.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Gutierrez, P.; Jana, D. K.; Marzin, A.; Meera-Lebbai, R.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Snow, J.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Khanov, A.; Rizatdinova, F.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Hamal, P.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Potter, C. T.; Ptacek, E.; Radloff, P.; Reinsch, A.; Searcy, J.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Andari, N.; Arnault, C.; Auge, E.; Barrillon, P.; Benoit, M.; Binet, S.; Bourdarios, C.; De la Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Matricon, P.; Niedercorn, F.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Ruan, X.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Teinturier, M.; Veillet, J. J.; Wicek, F.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Andari, N.; Arnault, C.; Auge, E.; Barrillon, P.; Benoit, M.; Binet, S.; Bourdarios, C.; De la Taille, C.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Idarraga, J.; Kado, M.; Martinez, N. Lorenzo; Lounis, A.; Makovec, N.; Matricon, P.; Niedercorn, F.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Ruan, X.; Rybkin, G.; Sauvan, J. B.; Schaarschmidt, J.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Teinturier, M.; Veillet, J. J.; Wicek, F.; Zerwas, D.; Zhang, Z.] IN2P3, CNRS, Orsay, France. [Hanagaki, K.; Hirose, M.; Lee, J. S. H.; Meguro, T.; Nomachi, M.; Sugaya, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Buran, T.; Cameron, D.; Gjelsten, B. K.; Lund, E.; Ould-Saada, F.; Pajchel, K.; Read, A. L.; Rohne, O.; Samset, B. H.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Apolle, R.; Barr, A. J.; Boddy, C. R.; Brandt, G.; Buchanan, J.; Buckingham, R. M.; Coniavitis, E.; Cooper-Sarkar, A. M.; Nca, A. Da Fi; Davies, E.; Gallas, E. J.; Gwenlan, C.; Hall, D.; Hays, C. P.; Howard, J.; Huffman, T. B.; Issever, C.; King, R. S. B.; Kogan, L. A.; Korn, A.; Larner, A.; Lewis, A.; Liang, Z.; Livermore, S. S. A.; Mattravers, C.; Nickerson, R. B.; Pinder, A.; Robichaud-Veronneau, A.; Ryder, N. C.; Short, D.; Tseng, J. C-L.; Vickey, T.; Viehhauser, G. H. A.; Weidberg, A. R.; Whitehead, S. R.; Young, C. J.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Colombo, T.; Conta, C.; Ferrari, R.; Franchino, S.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimodi, A.; Uslenghi, M.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Colombo, T.; Conta, C.; Franchino, S.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimodi, A.; Uslenghi, M.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Alison, J.; Brendlinger, K.; Degenhardt, J.; Fratina, S.; Hines, E.; Hong, T. M.; Jackson, B.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Olivito, D.; Ospanov, R.; Reece, R.; Saxon, J.; Schaefer, D.; Stahlman, J.; Thomson, E.; Wagner, P.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Bertolucci, F.; Cascella, M.; Cavasinni, V.; Crescioli, F.; Del Prete, T.; Dotti, A.; Roda, C.; Sarri, F.; White, S.; Zinonos, Z.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Bertolucci, F.; Cascella, M.; Cavasinni, V.; Crescioli, F.; Del Prete, T.; Dotti, A.; Roda, C.; Sarri, F.; White, S.; Zinonos, Z.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Boudreau, J.; Cleland, W.; Escobar, C.; Kittelmann, T.; Mueller, J.; Prieur, D.; Savinov, V.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amorim, A.; Anjos, N.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Do Valle Wemans, A.; Fiolhais, M. C. N.; Gomes, A.; Jorge, P. M.; Lopes, L.; Machado Miguens, J.; Maio, A.; Maneira, J.; Oliveira, M.; Onofre, A.; Palma, A.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Veloso, F.; Wolters, H.] LIP, Lab Instrumentacao & Fis Expt Particulas, P-1000 Lisbon, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Bohm, J.; Chudoba, J.; Gallus, P.; Gunther, J.; Jakoubek, T.; Juranek, V.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Marcisovsky, M.; Mikestikova, M.; Myska, M.; Nemecek, S.; Ruzicka, P.; Schovancova, J.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Tic, T.; Valenta, J.; Vrba, V.; Zeman, M.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Kodys, P.; Leitner, R.; Novakova, J.; Rybar, M.; Spousta, M.; Strachota, P.; Suk, M.; Sykora, T.; Tas, P.; Valkar, S.; Vorobe, V.; Wilhelm, I.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Augsten, K.; Holy, T.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Kral, V.; Krejci, F.; Pospisil, S.; Simak, V.; Slavicek, T.; Smolek, K.; Sodomka, J.; Solar, M.; Solc, J.; Sopko, V.; Sopko, B.; Stekl, I.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Ammosov, V. V.; Borisov, A.; Denisov, P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Ivashin, A. V.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.; Zmouchko, V. V.] Inst High Energy Phys, State Res Ctr, Protvino, Russia. [Adye, T.; Apolle, R.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Gillman, A. R.; Haywood, S. J.; Kirk, J.; Mattravers, C.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Nash, M.; Norton, P. R.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Strube, J.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Benslama, K.; Smit, C. V. Ybeles] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Artoni, G.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Pedis, D.; De Salvo, A.; De Zorzi, G.; Dionisi, C.; Falciano, S.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Rossi, E.; Tehrani, F. Safai; Sidoti, A.; Camillocci, E. Solfaroli; Vari, R.; Veneziano, S.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma 1, Rome, Italy. [Artoni, G.; Bagnaia, P.; Bini, C.; Caloi, R.; Ciapetti, G.; D'Orazio, A.; De Zorzi, G.; Dionisi, C.; Gauzzi, P.; Gentile, S.; Giagu, S.; Ippolito, V.; Lacava, F.; Lo Sterzo, F.; Luci, C.; Messina, A.; Rossi, E.; Camillocci, E. Solfaroli; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Di Simone, A.; Liberti, B.; Marchese, F.; Mazzaferro, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Cattani, G.; Di Ciaccio, A.; Di Simone, A.; Marchese, F.; Mazzaferro, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Branchini, P.; Ceradini, F.; Di Luise, S.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Stanescu, C.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Luise, S.; Orestano, D.; Pastore, F.; Petrucci, F.] Univ Roma Tre, Dipartimento Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.; Lablak, S.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA Marrakech, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Abreu, H.; Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Bolnet, N. M.; Boonekamp, M.; Chevalier, L.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Gauthier, L.; Giraud, P. F.; Guyot, C.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Legendre, M.; Maiani, C.; Mal, P.; Ramos, J. A. Manjarres; Mansoulie, B.; Meyer, J-P.; Mijovic, L.; Morange, N.; Mountricha, E.; Hong, V. Nguyen Thi; Nicolaidou, R.; Ouraou, A.; Resende, B.; Royon, C. R.; Schune, Ph; Schwindling, J.; Simard, O.; Virchaux, M.; Vranjes, N.; Xiao, M.; Xu, C.] CEA, CEA Saclay, DSM, IRFU Inst Rech Lois Fondamentales Univers, Gif Sur Yvette, France. [Chouridou, S.; Damiani, D. S.; Grillo, A. A.; Hare, G. A.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Mitrevski, J.; Nielsen, J.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Beckingham, M.; Coccaro, A.; Goussiou, A. G.; Harris, O. M.; Keller, J. S.; Lubatti, H. J.; Rompotis, N.; Rothberg, J.; Verducci, M.; Watts, G.; Zhao, T.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Booth, C. N.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Duxfield, R.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Mayne, A.; Mcfayden, J. A.; Miyagawa, P. S.; Owen, S.; Paganis, E.; Suruliz, K.; Tovey, D. R.; Tsionou, D.; Tua, A.; Xu, D.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Grybel, K.; Holder, M.; Ibragimov, I.; Rammes, M.; Rosenthal, O.; Sipica, V.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-5900 Siegen, Germany. [Dawe, E.; Godfrey, J.; Kvita, J.; O'Neil, D. C.; Petteni, M.; Stelzer, B.; Tanasijczuk, A. J.; Trottier-McDonald, M.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Butler, B.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Grenier, P.; Haas, A.; Hansson, P.; Jackson, P.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nelson, T. K.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Smith, D.; Strauss, E.; Su, D.; Wilson, M. G.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Batkova, L.; Blazek, T.; Federic, P.; Pecsy, M.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Ferencei, J.; Kladiva, E.; Seman, M.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Aurousseau, M.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Hamilton, A.; Leney, K. J. C.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Asman, B.; Bendtz, K.; Bohm, C.; Clement, C.; Eriksson, D.; Gellerstedt, K.; Hellman, S.; Holmgren, S. O.; Johansen, M.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Papadelis, A.; Sellden, B.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Asman, B.; Bendtz, K.; Clement, C.; Gellerstedt, K.; Hellman, S.; Johansen, M.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, J.; Lundberg, O.; Milstead, D. A.; Moa, T.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Yang, Z.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Ahmad, A.; Arfaoui, S.; Devetak, E.; DeWilde, B.; Engelmann, R.; Farley, J.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Ahmad, A.; Arfaoui, S.; Devetak, E.; DeWilde, B.; Engelmann, R.; Farley, J.; Goodson, J. J.; Grassi, V.; Gray, J. A.; Hobbs, J.; Jia, J.; Mastrandrea, P.; McCarthy, R. L.; Mohapatra, S.; Rijssenbeek, M.; Schamberger, R. D.; Stupak, J.; Tsybychev, D.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Bartsch, V.; De Santo, A.; Martin-Haugh, S.; Potter, C. J.; Rose, A.; Salvatore, F.; Sutton, M. R.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Bangert, A.; Cuthbert, C.; Patel, N.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Waugh, A. T.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Chu, M. L.; Hou, S.; Lee, S. C.; Lin, S. C.; Liu, D.; Mazini, R.; Meng, Z.; Ren, Z. L.; Soh, D. A.; Teng, P. K.; Wang, H.; Wang, J.; Wang, S. M.; Weng, Z.; Zhang, D.; Zhou, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Harpaz, S. Behar; Kajomovitz, E.; Rozen, Y.; Tarem, S.; Vallecorsa, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Bella, G.; Benary, O.; Benhammou, Y.; Etzion, E.; Gershon, A.; Ginzburg, J.; Guttman, N.; Hod, N.; Munwes, Y.; Oren, Y.; Reinherz-Aronis, E.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Iliadis, D.; Kordas, K.; Kouskoura, V.; Nomidis, I.; Petridis, A.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, K.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yamazaki, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Matsunaga, H.; Nakamura, K.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yamazaki, T.] Univ Tokyo, Dept Phys, Tokyo 113, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Ishitsuka, M.; Jinnouchi, O.; Kanno, T.; Kuze, M.; Nagai, R.; Nobe, T.] Tokyo Inst Technol, Dept Phys, Tokyo 152, Japan. [AbouZeid, O. S.; Bailey, D. C.; Bain, T.; Brelier, B.; Cheung, S. L.; Dhaliwal, S.; Farooque, T.; Fatholahzadeh, B.; Gibson, A.; Guo, B.; Ilic, N.; Keung, J.; Knecht, N. S.; Krieger, P.; Le Maner, C.; Martens, F. K.; Orr, R. S.; Rezvani, R.; Rosenbaum, G. A.; Savard, P.; Sinervo, P.; Spreitzer, T.; Tardif, D.; Teuscher, R. J.; Thompson, P. D.; Trischuk, W.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Fortin, D.; Gingrich, D. M.; Koutsman, A.; Losty, M. J.; Nugent, I. M.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schouten, D.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hanawa, K.; Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Kurata, M.; Nagai, K.; Ukegawa, F.] Univ Tsukuba, Inst Pure & Appl Sci, Tsukuba, Ibaraki 3058571, Japan. [Beauchemin, P. H.; Hamilton, S.; Meoni, E.; Napier, A.; Rolli, S.; Sliwa, K.; Todorova-Nova, S.; Wetter, J.] Tufts Univ, Ctr Sci & Technol, Medford, MA 02155 USA. [Losada, M.; Loureiro, K. F.; Mendoza Navas, L.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, uniant, Bogota, Colombia. [Avolio, G.; Deng, J.; Farrell, S.; Eschrich, I. Gough; Hawkins, D.; Lankford, A. J.; Magnoni, L.; Mete, A. S.; Nelson, A.; Scannicchio, D. A.; Schernau, M.; Taffard, A.; Toggerson, B.; Unel, G.; Werth, M.; Wheeler-Ellis, S. J.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Del Papa, C.; Giordani, M. P.; Pinamonti, M.; Shaw, K.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Acharya, B. S.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Acharya, B. S.; Alhroob, M.; Brazzale, S. F.; Cobal, M.; De Sanctis, U.; Del Papa, C.; Pinamonti, M.; Shaw, K.; Soualah, R.] Ist Nazl Fis Nucl, Grp Collegato Udine, Udine, Italy. [Atkinson, M.; Basye, A.; Benekos, N.; Cavaliere, V.; Chang, P.; Coggeshall, J.; Cortes-Gonzalez, A.; Errede, D.; Errede, S.; Lie, K.; Liss, T. M.; McCarn, A.; Neubauer, M. S.; Vichou, I.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Brenner, R.; Buszello, C. P.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Pelikan, D.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Urban, S. Cabrera; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] CSIC, Valencia, Spain. [Urban, S. Cabrera; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Urban, S. Cabrera; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Urban, S. Cabrera; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Urban, S. Cabrera; Castillo Gimenez, V.; Costa, M. J.; Fassi, F.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Kaci, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Moya, M. Minano; Mitsou, V. A.; Moles-Valls, R.; Moreno Llacer, M.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez Martinez, V.; Solans, C. A.; Soldevila, U.; Sanchez, J.; Torro Pastor, E.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Villaplana Perez, M.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Axen, D.; Gay, C.; Gecse, Z.; Loh, C. W.; Mills, W. J.; Swedish, S.; Viel, S.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Astbury, A.; Bansal, V.; Berghaus, F.; Courneyea, L.; Fincke-Keeler, M.; Keeler, R.; Kowalewski, R.; Lefebvre, M.; Lessard, J-R.; Marino, C. P.; Martyniuk, A. C.; McPherson, R. A.; Ouellette, E. A.; Plamondon, M.; Sobie, R.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Farrington, S. M.; Jones, G.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Kimura, N.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Alon, R.; Barak, L.; Bressler, S.; Duchovni, E.; Frank, T.; Gabizon, O.; Gross, E.; Groth-Jensen, J.; Klier, A.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Milstein, D.; Roth, I.; Silbert, O.; Smakhtin, V.; Vitells, O.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Asfandiyarov, R.; Banerjee, Sw; Montoya, G. D. Carrillo; Hernandez, A. M. Castaneda; Castaneda-Miranda, E.; Chen, X.; Di Mattia, A.; Dos Anjos, A.; Fang, Y.; Castillo, L. R. Flores; Gonzalez, S.; Gutzwiller, O.; Ji, H.; Ju, X.; Kashif, L.; Li, H.; Ma, L. L.; Garcia, B. R. Mellado; Ming, Y.; Pan, Y. B.; Morales, M. I. Pedraza; Quayle, W. B.; Sarangi, T.; Wang, H.; Wiedenmann, W.; Wu, S. L.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Fleischmann, P.; Meyer, J.; Redelbach, A.; Siragusa, G.; Stroehmer, R.; Trefzger, T.] Univ Wurzburg, Fak Phys & Astron, Wurzburg, Germany. [Barisonzi, M.; Becker, A. K.; Becks, K. H.; Boek, J.; Braun, H. M.; Cornelissen, T.; Duda, D.; Fleischmann, S.; Flick, T.; Gerlach, P.; Glitza, K. W.; Gorfine, G.; Hamacher, K.; Harenberg, T.; Henss, T.; Hirschbuehl, D.; Kalinin, S.; Kersten, S.; Khoroshilov, A.; Kohlmann, S.; Lantzsch, K.; Lenzen, G.; Maettig, P.; Mechtel, M.; Neumann, M.; Pataraia, S.; Sandhoff, M.; Sartisohn, G.; Schultes, J.; Sturm, P.; Voss, T. T.; Wagner, W.; Wahlen, H.; Wicke, D.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich Phys C, Wuppertal, Germany. [Adelman, J.; Baker, O. K.; Bedikian, S.; Almenar, C. Cuenca; Czyczula, Z.; Demers, S.; Garberson, F.; Golling, T.; Guest, D.; Lee, L.; Loginov, A.; Sherman, D.; Tipton, P.; Wall, R.; Walsh, B.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Biscarat, C.; Cogneras, E.; Rahal, G.] IN2P3, CNRS, Ctr Calcul, Villeurbanne, France. [Amorim, A.; Gomes, A.; Maio, A.; Pina, J.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amorim, A.; Gomes, A.; Maio, A.; Pina, J.] Univ Lisbon, CFNUL, Lisbon, Portugal. [Bawa, H. S.; Gao, Y. S.; Lowe, A. J.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beloborodova, O.; Talyshev, A.; Tikhonov, Y. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Canelli, F.] Fermilab Natl Accelerator Lab, Batavia, IL USA. [Carvalho, J.; Fiolhais, M. C. N.; Oliveira, M.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Hernandez, A. M. Castaneda] UASLP, Dept Phys, San Luis Potosi, Mexico. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Demirkoz, B.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Dhullipudi, R.; Greenwood, Z. D.; Sawyer, L.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Do Valle Wemans, A.] Univ Nova Lisboa, Dep Fis, Caparica, Portugal. [Do Valle Wemans, A.] Univ Nova Lisboa, CEFITEC Fac Ciencias & Tecnol, Caparica, Portugal. [Guler, H.] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Kono, T.; Wildt, M. A.] Univ Hamburg, Inst Expt Phys, Hamburg, Germany. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Li, H.; Meng, Z.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Liang, Z.; Soh, D. A.; Weng, Z.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou, Peoples R China. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Park, W.; Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Pasztor, G.; Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Perez, K.] CALTECH, Pasadena, CA 91125 USA. [Richter-Was, E.] Jagiellonian Univ, Inst Phys, Krakow, Poland. [Yacoob, S.] Univ KwaZulu Natal, Discipline Phys, Durban, South Africa. RP Aad, G (reprint author), Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. RI Conde Muino, Patricia/F-7696-2011; Andreazza, Attilio/E-5642-2011; Boyko, Igor/J-3659-2013; Kuleshov, Sergey/D-9940-2013; Anjos, Nuno/I-3918-2013; Kartvelishvili, Vakhtang/K-2312-2013; Dawson, Ian/K-6090-2013; Solfaroli Camillocci, Elena/J-1596-2012; Tudorache, Alexandra/L-3557-2013; Tudorache, Valentina/D-2743-2012; Marti-Garcia, Salvador/F-3085-2011; Wolters, Helmut/M-4154-2013; Ma, Hong/F-2725-2011; Orlov, Ilya/E-6611-2012; Petrucci, Fabrizio/G-8348-2012; Annovi, Alberto/G-6028-2012; Stoicea, Gabriel/B-6717-2011; Brooks, William/C-8636-2013; Pina, Joao /C-4391-2012; Amorim, Antonio/C-8460-2013; Vanyashin, Aleksandr/H-7796-2013; Casadei, Diego/I-1785-2013; La Rosa, Alessandro/I-1856-2013; Moraes, Arthur/F-6478-2010; Smirnov, Sergei/F-1014-2011; Ferrando, James/A-9192-2012; Veneziano, Stefano/J-1610-2012; Wemans, Andre/A-6738-2012; Doyle, Anthony/C-5889-2009; Alexa, Calin/F-6345-2010; Gutierrez, Phillip/C-1161-2011; Fazio, Salvatore /G-5156-2010; Bergeaas Kuutmann, Elin/A-5204-2013; Cascella, Michele/B-6156-2013; messina, andrea/C-2753-2013; Weigell, Philipp/I-9356-2012; de Groot, Nicolo/A-2675-2009; Moorhead, Gareth/B-6634-2009; Fassi, Farida/F-3571-2016; la rotonda, laura/B-4028-2016; Korol, Aleksandr/A-6244-2014; Karyukhin, Andrey/J-3904-2014; Capua, Marcella/A-8549-2015; Tartarelli, Giuseppe Francesco/A-5629-2016; Mora Herrera, Maria Clemencia/L-3893-2016; Maneira, Jose/D-8486-2011; KHODINOV, ALEKSANDR/D-6269-2015; Goncalo, Ricardo/M-3153-2016; Gauzzi, Paolo/D-2615-2009; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Martinez, Mario /I-3549-2015; Yang, Haijun/O-1055-2015; Monzani, Simone/D-6328-2017; Grancagnolo, Francesco/K-2857-2015; Gonzalez de la Hoz, Santiago/E-2494-2016; Guo, Jun/O-5202-2015; Smirnova, Oxana/A-4401-2013; Aguilar Saavedra, Juan Antonio/F-1256-2016; Leyton, Michael/G-2214-2016; Jones, Roger/H-5578-2011; Vranjes Milosavljevic, Marija/F-9847-2016; SULIN, VLADIMIR/N-2793-2015; Nechaeva, Polina/N-1148-2015; Olshevskiy, Alexander/I-1580-2016; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Grancagnolo, Sergio/J-3957-2015; spagnolo, stefania/A-6359-2012; Shmeleva, Alevtina/M-6199-2015; Camarri, Paolo/M-7979-2015; Gavrilenko, Igor/M-8260-2015; Tikhomirov, Vladimir/M-6194-2015; Chekulaev, Sergey/O-1145-2015; Gorelov, Igor/J-9010-2015; Gladilin, Leonid/B-5226-2011; Carvalho, Joao/M-4060-2013; Mashinistov, Ruslan/M-8356-2015; Booth, Christopher/B-5263-2016; Ventura, Andrea/A-9544-2015; Livan, Michele/D-7531-2012; Mitsou, Vasiliki/D-1967-2009; Joergensen, Morten/E-6847-2015; Riu, Imma/L-7385-2014; Mir, Lluisa-Maria/G-7212-2015; Garcia, Jose /H-6339-2015; Della Pietra, Massimo/J-5008-2012; Cavalli-Sforza, Matteo/H-7102-2015; Ferrer, Antonio/H-2942-2015; Prokoshin, Fedor/E-2795-2012; Hansen, John/B-9058-2015; Staroba, Pavel/G-8850-2014; Kupco, Alexander/G-9713-2014; Mikestikova, Marcela/H-1996-2014; Kuday, Sinan/C-8528-2014; Snesarev, Andrey/H-5090-2013; Svatos, Michal/G-8437-2014; Chudoba, Jiri/G-7737-2014; Peleganchuk, Sergey/J-6722-2014; Santamarina Rios, Cibran/K-4686-2014; Bosman, Martine/J-9917-2014; Lei, Xiaowen/O-4348-2014; Demirkoz, Bilge/C-8179-2014; Warburton, Andreas/N-8028-2013; De, Kaushik/N-1953-2013; Sukharev, Andrey/A-6470-2014; O'Shea, Val/G-1279-2010; Lee, Jason/B-9701-2014; Robson, Aidan/G-1087-2011; Negrini, Matteo/C-8906-2014; Fabbri, Laura/H-3442-2012; Villa, Mauro/C-9883-2009; Kepka, Oldrich/G-6375-2014; Nemecek, Stanislav/G-5931-2014; Jakoubek, Tomas/G-8644-2014; Lokajicek, Milos/G-7800-2014 OI Conde Muino, Patricia/0000-0002-9187-7478; Andreazza, Attilio/0000-0001-5161-5759; Boyko, Igor/0000-0002-3355-4662; Kuleshov, Sergey/0000-0002-3065-326X; Solfaroli Camillocci, Elena/0000-0002-5347-7764; Wolters, Helmut/0000-0002-9588-1773; Orlov, Ilya/0000-0003-4073-0326; Petrucci, Fabrizio/0000-0002-5278-2206; Annovi, Alberto/0000-0002-4649-4398; Stoicea, Gabriel/0000-0002-7511-4614; Brooks, William/0000-0001-6161-3570; Pina, Joao /0000-0001-8959-5044; Vanyashin, Aleksandr/0000-0002-0367-5666; La Rosa, Alessandro/0000-0001-6291-2142; Moraes, Arthur/0000-0002-5157-5686; Smirnov, Sergei/0000-0002-6778-073X; Ferrando, James/0000-0002-1007-7816; Veneziano, Stefano/0000-0002-2598-2659; Wemans, Andre/0000-0002-9669-9500; Doyle, Anthony/0000-0001-6322-6195; Cascella, Michele/0000-0003-2091-2501; Moorhead, Gareth/0000-0002-9299-9549; Doria, Alessandra/0000-0002-5381-2649; Veloso, Filipe/0000-0002-5956-4244; Gomes, Agostinho/0000-0002-5940-9893; Fassi, Farida/0000-0002-6423-7213; la rotonda, laura/0000-0002-6780-5829; Osculati, Bianca Maria/0000-0002-7246-060X; Amorim, Antonio/0000-0003-0638-2321; Santos, Helena/0000-0003-1710-9291; Coccaro, Andrea/0000-0003-2368-4559; Korol, Aleksandr/0000-0001-8448-218X; Maio, Amelia/0000-0001-9099-0009; Fiolhais, Miguel/0000-0001-9035-0335; Karyukhin, Andrey/0000-0001-9087-4315; Anjos, Nuno/0000-0002-0018-0633; Giordani, Mario/0000-0002-0792-6039; Abdelalim, Ahmed Ali/0000-0002-2056-7894; Capua, Marcella/0000-0002-2443-6525; Di Micco, Biagio/0000-0002-4067-1592; Tartarelli, Giuseppe Francesco/0000-0002-4244-502X; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Maneira, Jose/0000-0002-3222-2738; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Goncalo, Ricardo/0000-0002-3826-3442; Gauzzi, Paolo/0000-0003-4841-5822; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Monzani, Simone/0000-0002-0479-2207; Grancagnolo, Francesco/0000-0002-9367-3380; Gonzalez de la Hoz, Santiago/0000-0001-5304-5390; Guo, Jun/0000-0001-8125-9433; Smirnova, Oxana/0000-0003-2517-531X; Aguilar Saavedra, Juan Antonio/0000-0002-5475-8920; Leyton, Michael/0000-0002-0727-8107; Jones, Roger/0000-0002-6427-3513; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; SULIN, VLADIMIR/0000-0003-3943-2495; Olshevskiy, Alexander/0000-0002-8902-1793; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Grancagnolo, Sergio/0000-0001-8490-8304; spagnolo, stefania/0000-0001-7482-6348; Camarri, Paolo/0000-0002-5732-5645; Tikhomirov, Vladimir/0000-0002-9634-0581; Gorelov, Igor/0000-0001-5570-0133; Gladilin, Leonid/0000-0001-9422-8636; Carvalho, Joao/0000-0002-3015-7821; Mashinistov, Ruslan/0000-0001-7925-4676; Booth, Christopher/0000-0002-6051-2847; Ventura, Andrea/0000-0002-3368-3413; Livan, Michele/0000-0002-5877-0062; Mitsou, Vasiliki/0000-0002-1533-8886; Joergensen, Morten/0000-0002-6790-9361; Riu, Imma/0000-0002-3742-4582; Mir, Lluisa-Maria/0000-0002-4276-715X; Della Pietra, Massimo/0000-0003-4446-3368; Ferrer, Antonio/0000-0003-0532-711X; Prokoshin, Fedor/0000-0001-6389-5399; Hansen, John/0000-0002-8422-5543; Mikestikova, Marcela/0000-0003-1277-2596; Kuday, Sinan/0000-0002-0116-5494; Svatos, Michal/0000-0002-7199-3383; Peleganchuk, Sergey/0000-0003-0907-7592; Santamarina Rios, Cibran/0000-0002-9810-1816; Bosman, Martine/0000-0002-7290-643X; Lei, Xiaowen/0000-0002-2564-8351; Warburton, Andreas/0000-0002-2298-7315; De, Kaushik/0000-0002-5647-4489; O'Shea, Val/0000-0001-7183-1205; Lee, Jason/0000-0002-2153-1519; Negrini, Matteo/0000-0003-0101-6963; Fabbri, Laura/0000-0002-4002-8353; Villa, Mauro/0000-0002-9181-8048; FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; EPLANET, European Union; ERC, European Union; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; DFG, Germany; HGF, Germany; MPG, Germany; AvH Foundation, Germany; GSRT, Greece; ISF, Israel; MINERVA, Israel; GIF, Israel; DIP, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; GRICES, Portugal; FCT, Portugal; MERYS (MECTS), Romania; MES of Russia, Russian Federation; ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MVZT, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SER, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, United Kingdom; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; DOE, United States of America; NSF, United States of America FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; EPLANET and ERC, European Union; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, DFG, HGF, MPG and AvH Foundation, Germany; GSRT, Greece; ISF, MINERVA, GIF, DIP and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW, Poland; GRICES and FCT, Portugal; MERYS (MECTS), Romania; MES of Russia and ROSATOM, Russian Federation; JINR; MSTD, Serbia; MSSR, Slovakia; ARRS and MVZT, Slovenia; DST/NRF, South Africa; MICINN, Spain; SRC and Wallenberg Foundation, Sweden; SER, SNSF and Cantons of Bern and Geneva, Switzerland; NSC, Taiwan; TAEK, Turkey; STFC, the Royal Society and Leverhulme Trust, United Kingdom; DOE and NSF, United States of America. NR 47 TC 2 Z9 2 U1 4 U2 97 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD NOV PY 2012 IS 11 AR 033 DI 10.1007/JHEP11(2012)033 PG 54 WC Physics, Particles & Fields SC Physics GA 052KZ UT WOS:000312197800033 ER PT J AU Abelev, B Adam, J Adamova, D Adare, AM Aggarwal, M Rinella, GA Agocs, AC Agostinelli, A Salazar, SA Ahammed, Z Ahmad, A Ahmad, N Ahn, SA Ahn, SU Akindinov, A Aleksandrov, D Alessandro, B Molina, JRA Alici, A Alkin, A Avina, EJA Alme, J Alt, T Altini, V Altinpinar, S Altsybeev, I Andrei, C Andronic, A Anguelov, V Anielski, J Anson, CD Anticic, T Antinori, F Antonioli, P Aphecetche, LB Appelshauser, H Arbor, N Arcelli, S Arend, A Armesto, N Arnaldi, R Aronsson, TR Arsene, IC Arslandok, M Asryan, A Augustinus, A Averbeck, RP Awes, T Aysto, JH Azmi, MD Bach, MJ Badala, A Baek, YW Bailhache, RM Bala, R Ferroli, RB Baldisseri, A Baldit, A Pedrosa, FBD Ban, J Baral, RC Barbera, R Barile, F Barnafoldi, GG Barnby, LS Barret, V Bartke, JG Basile, M Bastid, N Basu, S Bathen, B Batigne, G Batyunya, B Baumann, CH Bearden, IG Beck, H Behera, NK Belikov, I Bellini, F Bellwied, R Belmont-Moreno, E Bencedi, G Beole, S Berceanu, I Bercuci, A Berdnikov, Y Berenyi, D Bergognon, AAE Berzano, D Betev, L Bhasin, A Bhati, AK Bhom, J Bianchi, L Bianchi, N Bianchin, C Bielcik, J Bielcikova, J Bilandzic, A Bjelogrlic, S Blanco, F Blanco, F Blau, D Blume, C Boccioli, M Bock, N Boettger, S Bogdanov, A Boggild, H Bogolyubsky, M Boldizsar, L Bombara, M Book, J Borel, H Borissov, A Bose, SN Bossu, F Botje, M Boyer, BA Braidot, E Braun-Munzinger, P Bregant, M Breitner, TG Browning, TA Broz, M Brun, R Bruna, E Bruno, GE Budnikov, D Buesching, H Bufalino, S Bugaiev, K Busch, O Buthelezi, EZ Orduna, DC Caffarri, D Cai, X Caines, HL Villar, EC Camerini, P Roman, VC Romeo, GC Carena, F Carena, W Carlin, N Carminati, F Montoya, CAC Diaz, AOC Castellanos, JEC Hernandez, JFC Casula, EAR Catanescu, V Cavicchioli, C Sanchez, CC Cepila, J Cerello, P Chang, B Chapeland, S Charvet, JLF Chattopadhyay, S Chattopadhyay, S Chawla, I Cherney, MG Cheshkov, C Cheynis, B Barroso, VMC Chinellato, D Chochula, P Chojnacki, M Choudhury, S Christakoglou, P Christensen, CH Christiansen, P Chujo, T Chung, SU Cicalo, C Cifarelli, L Cindolo, F Cleymans, JWA Coccetti, F Colamaria, F Colella, D Balbastre, GC del Valle, ZC Constantin, P Contin, G Contreras, JG Cormier, TM Morales, YC Cortese, P Maldonado, IC Cosentino, MR Costa, F Cotallo, ME Crescio, E Crochet, P Alaniz, EC Cuautle, E Cunqueiro, L Dainese, A Dalsgaard, HH Danu, A Das, D Das, I Das, K Dash, S Dash, AK De, S de Barros, G De Caro, A de Cataldo, G de Cuveland, J De Falco, A De Gruttola, D Delagrange, H Deloff, A Demanov, V De Marco, N Denes, E De Pasquale, S Deppman, A D'Erasmo, G de Rooij, RS Corchero, MAD Di Bari, D Di Giglio, C Dietel, T Di Liberto, S Di Mauro, A Di Nezza, P Divia, R Djuvsland, O Dobrin, AF Dobrowolski, TA Dominguez, I Donigus, B Dordic, O Driga, O Dubey, AK Ducroux, L Dupieux, P Majumdar, MRD Majumdar, AKD Elia, D Emschermann, DP Engel, H Erdal, HA Espagnon, B Estienne, MD Esumi, 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B. Kurepin, A. Kuryakin, Alexey Kushpil, Vasily Kushpil, Svetlana Kvaerno, Henning Kweon, Min Jung Kwon, Youngil Ladron de Guevara, Pedro Lakomov, Igor Langoy, Rune La Pointe, Sarah Louise Lara, Camilo Ernesto Lardeux, Antoine Xavier La Rocca, Paola Lazzeroni, Cristina Lea, Ramona Le Bornec, Yves Lechman, Mateusz Lee, Sung Chul Lee, Ki Sang Lee, Graham Richard Lefevre, Frederic Lehnert, Joerg Walter Leistam, Lars Lenhardt, Matthieu Laurent Lenti, Vito Leon, Hermes Leoncino, Marco Leon Monzon, Ildefonso Vargas, Hermes Leon Levai, Peter Lien, Jorgen Lietava, Roman Lindal, Svein Lindenstruth, Volker Lippmann, Christian Lisa, Michael Annan Liu, Lijiao Loenne, Per-Ivar Loggins, Vera Loginov, Vitaly Lohn, Stefan Bernhard Lohner, Daniel Loizides, Constantinos Loo, Kai Krister Lopez, Xavier Bernard Lopez Torres, Ernesto Lovhoiden, Gunnar Lu, Xianguo Luettig, Philipp Lunardon, Marcello Luo, Jiebin Luparello, Grazia Luquin, Lionel Luzzi, Cinzia Ma, Rongrong Ma, Ke Madagodahettige-Don, Dilan Minthaka Maevskaya, Alla Mager, Magnus Mahapatra, Durga Prasad Maire, Antonin Malaev, Mikhail Maldonado Cervantes, Ivonne Alicia Malinina, Ludmila Mal'Kevich, Dmitry Malzacher, Peter Mamonov, Alexander Manceau, Loic Henri Antoine Mangotra, Lalit Kumar Manko, Vladislav Manso, Franck Manzari, Vito Mao, Yaxian Marchisone, Massimiliano Mares, Jiri Margagliotti, Giacomo Vito Margotti, Anselmo Marin, Ana Maria Tobon, Cesar Augusto Marin Markert, Christina Martashvili, Irakli Martinengo, Paolo Martinez, Mario Ivan Davalos, Arnulfo Martinez Garcia, Gines Martinez Martynov, Yevgen Mas, Alexis Jean-Michel Masciocchi, Silvia Masera, Massimo Masoni, Alberto Massacrier, Laure Marie Mastromarco, Mario Mastroserio, Annalisa Matthews, Zoe Louise Matyja, Adam Tomasz Mayani, Daniel Mayer, Christoph Mazer, Joel Mazzoni, Alessandra Maria Meddi, Franco Alejandro Menchaca-Rocha, Arturo Perez, Jorge Mercado Meres, Michal Miake, Yasuo Milano, Leonardo Milosevic, Jovan Mischke, Andre Mishra, Aditya Nath Miskowiec, Dariusz Mitu, Ciprian Mihai Mlynarz, Jocelyn Mohanty, Bedangadas Mohanty, Ajit Kumar Molnar, Levente Montano Zetina, Luis Manuel Monteno, Marco Montes, Esther Moon, Taebong Morando, Maurizio Moreira De Godoy, Denise Aparecida Moretto, Sandra Morsch, Andreas Muccifora, Valeria Mudnic, Eugen Muhuri, Sanjib Mukherjee, Maitreyee Muller, Hans Munhoz, Marcelo Musa, Luciano Musso, Alfredo Nandi, Basanta Kumar Nania, Rosario Nappi, Eugenio Nattrass, Christine Naumov, Nikolay Navin, Sparsh Nayak, Tapan Kumar Nazarenko, Sergey Nazarov, Gleb Nedosekin, Alexander Nicassio, Maria Niculescu, Mihai Nielsen, Borge Svane Niida, Takafumi Nikolaev, Sergey Nikolic, Vedran Nikulin, Sergey Nikulin, Vladimir Nilsen, Bjorn Steven Nilsson, Mads Stormo Noferini, Francesco Nomokonov, Petr Nooren, Gerardus Novitzky, Norbert Nyanin, Alexandre Nyatha, Anitha Nygaard, Casper Nystrand, Joakim Ingemar Ochirov, Alexander Oeschler, Helmut Oskar Oh, Saehanseul Oh, Sun Kun Oleniacz, Janusz Oppedisano, Chiara Velasquez, Antonio Ortiz Ortona, Giacomo Oskarsson, Anders Nils Erik Ostrowski, Piotr Krystian Otwinowski, Jacek Tomasz Oyama, Ken Ozawa, Kyoichiro Pachmayer, Yvonne Chiara Pachr, Milos Padilla, Fatima Pagano, Paola Paic, Guy Painke, Florian Pajares, Carlos Pal, S. Pal, Susanta Kumar Palaha, Arvinder Singh Palmeri, Armando Papikyan, Vardanush Pappalardo, Giuseppe Park, Woo Jin Passfeld, Annika Pastircak, Blahoslav Patalakha, Dmitri Ivanovich Paticchio, Vincenzo Pavlinov, Alexei Pawlak, Tomasz Jan Peitzmann, Thomas Da Costa, Hugo Denis Antonio Pereira De Oliveira Filho, Elienos Pereira Peresunko, Dmitri Lara, Carlos Eugenio Perez Lezama, Edgar Perez Perini, Diego Perrino, Davide Peryt, Wiktor Stanislaw Pesci, Alessandro Peskov, Vladimir Pestov, Yury Petracek, Vojtech Petran, Michal Petris, Mariana Petrov, Plamen Rumenov Petrovici, Mihai Petta, Catia Piano, Stefano Piccotti, Anna Pikna, Miroslav Pillot, Philippe Pinazza, Ombretta Pinsky, Lawrence Pitz, Nora Piyarathna, Danthasinghe Ploskon, Mateusz Andrzej Pluta, Jan Marian Pocheptsov, Timur Pochybova, Sona Podesta Lerma, Pedro Luis Manuel Poghosyan, Martin Polak, Karel Polichtchouk, Boris Pop, Amalia Porteboeuf-Houssais, Sarah Pospisil, Vladimir Potukuchi, Baba Prasad, Sidharth Kumar Preghenella, Roberto Prino, Francesco Pruneau, Claude Andre Pshenichnov, Igor Puchagin, Sergey Puddu, Giovanna Teixido, Jordi Pujol Pulvirenti, Alberto Punin, Valery Putis, Marian Putschke, Jorn Henning Quercigh, Emanuele Qvigstad, Henrik Rachevski, Alexandre Rademakers, Alphonse Radomski, Sylwester Raiha, Tomi Samuli Rak, Jan Rakotozafindrabe, Andry Malala Ramello, Luciano Ramirez Reyes, Abdiel Raniwala, Sudhir Raniwala, Rashmi Rasanen, Sami Sakari Rascanu, Bogdan Theodor Rathee, Deepika Read, Kenneth Francis Real, Jean-Sebastien Redlich, Krzysztof Reichelt, Patrick Reicher, Martijn Renfordt, Rainer Arno Ernst Reolon, Anna Rita Reshetin, Andrey Rettig, Felix Vincenz Revol, Jean-Pierre Reygers, Klaus Johannes Riccati, Lodovico Ricci, Renato Angelo Richert, Tuva Richter, Matthias Rudolph Riedler, Petra Riegler, Werner Riggi, Francesco Rabacal, Bartolomeu Rodrigues Fernandes Rodriguez Cahuantzi, Mario Manso, Alis Rodriguez Roed, Ketil Rohr, David Rohrich, Dieter Romita, Rosa Ronchetti, Federico Rosnet, Philippe Rossegger, Stefan Rossi, Andrea Roy, Christelle Sophie Roy, Pradip Kumar Rubio Montero, Antonio Juan Rui, Rinaldo Ryabinkin, Evgeny Rybicki, Andrzej Sadovsky, Sergey Safarik, Karel Sahoo, Raghunath Sahu, Pradip Kumar Saini, Jogender Sakaguchi, Hiroaki Sakai, Shingo Sakata, Dosatsu Albert Salgado, Carlos Salzwedel, Jai Sambyal, Sanjeev Singh Samsonov, Vladimir Castro, Xitzel Sanchez Sandor, Ladislav Sandoval, Andres Sano, Satoshi Sano, Masato Santo, Rainer Santoro, Romualdo Sarkamo, Juho Jaako Scapparone, Eugenio Scarlassara, Fernando Scharenberg, Rolf Paul Schiaua, Claudiu Cornel Schicker, Rainer Martin Schmidt, Christian Joachim Schmidt, Hans Rudolf Schreiner, Steffen Schuchmann, Simone Schukraft, Jurgen Schutz, Yves Roland Schwarz, Kilian Eberhard Schweda, Kai Oliver Scioli, Gilda Scomparin, Enrico Scott, Rebecca Scott, Patrick Aaron Segato, Gianfranco Selioujenkov, Ilya Senyukov, Serhiy Seo, Jeewon Serci, Sergio Serradilla, Eulogio Sevcenco, Adrian Shabetai, Alexandre Shabratova, Galina Shahoyan, Ruben Sharma, Natasha Sharma, Satish Sharma, Rohini Shigaki, Kenta Shimomura, Maya Shtejer, Katherin Sibiriak, Yury Siciliano, Melinda Sicking, Eva Siddhanta, Sabyasachi Siemiarczuk, Teodor Silvermyr, David Olle Rickard Silvestre, Catherine Simatovic, Goran Simonetti, Giuseppe Singaraju, Rama Narayana Singh, Ranbir Singha, Subhash Singhal, Vikas Sinha, Tinku Sinha, Bikash Sitar, Branislav Sitta, Mario Skaali, Bernhard Skjerdal, Kyrre Smakal, Radek Smirnov, Nikolai Snellings, Raimond Sogaard, Carsten Soltz, Ron Ariel Son, Hyungsuk Song, Myunggeun Song, Jihye Soos, Csaba Soramel, Francesca Sputowska, Iwona Spyropoulou-Stassinaki, Martha Srivastava, Brijesh Kumar Stachel, Johanna Stan, Ionel Stan, Ionel Stefanek, Grzegorz Steinbeck, Timm Morten Steinpreis, Matthew Stenlund, Evert Anders Steyn, Gideon Francois Stiller, Johannes Hendrik Stocco, Diego Stolpovskiy, Mikhail Strabykin, Kirill Strmen, Peter do Passo Suaide, Alexandre Alarcon Vasquez, Martin Alfonso Subieta Sugitate, Toru Suire, Christophe Pierre Sukhorukov, Mikhail Sultanov, Rishat Sumbera, Michal Susa, Tatjana de Toledo, Alejandro Szanto Szarka, Imrich Szczepankiewicz, Adam Szostak, Artur Krzysztof Szymanski, Maciej Takahashi, Jun Takaki, Daniel Jesus Tapia Tauro, Arturo Tejeda Munoz, Guillermo Telesca, Adriana Terrevoli, Cristina Thader, Jochen Mathias Thomas, Deepa Tieulent, Raphael Noel Timmins, Anthony Tlusty, David Toia, Alberica Torii, Hisayuki Toscano, Luca Truesdale, David Christopher Trzaska, Wladyslaw Henryk Tsuji, Tomoya Tumkin, Alexandr Turrisi, Rosario Tveter, Trine Spedstad Ulery, Jason Glyndwr Ullaland, Kjetil Ulrich, Jochen Uras, Antonio Urban, Jozef Urciuoli, Guido Marie Usai, Gianluca Vajzer, Michal Vala, Martin Palomo, Lizardo Valencia Vallero, Sara van der Kolk, Naomi Vyvre, Pierre Vande van Leeuwen, Marco Vannucci, Luigi Diozcora Vargas, Aurora Varma, Raghava Vasileiou, Maria Vasiliev, Andrey Vechernin, Vladimir Veldhoen, Misha Venaruzzo, Massimo Vercellin, Ermanno Vergara, Sergio Vernet, Renaud Verweij, Marta Vickovic, Linda Viesti, Giuseppe Vikhlyantsev, Oleg Vilakazi, Zabulon Baillie, Orlando Villalobos Vinogradov, Alexander Vinogradov, Leonid Vinogradov, Yury Virgili, Tiziano Viyogi, Yogendra Vodopianov, Alexander Voloshin, Kirill Voloshin, Sergey Volpe, Giacomo von Haller, Barthelemy Vranic, Danilo Vrebekk, Gaute Vrlakova, Janka Vulpescu, Bogdan Vyushin, Alexey Wagner, Vladimir Wagner, Boris Wan, Renzhuo Wang, Mengliang Wang, Dong Wang, Yifei Wang, Yaping Watanabe, Kengo Weber, Michael Wessels, Johannes Westerhoff, Uwe Wiechula, Jens Wikne, Jon Wilde, Martin Rudolf Wilk, Grzegorz Andrzej Wilk, Alexander Williams, Crispin Windelband, Bernd Stefan Karampatsos, Leonidas Xaplanteris Yaldo, Chris G. Yamaguchi, Yorito Yang, Hongyan Yang, Shiming Yasnopolsky, Stanislav Yi, JunGyu Yin, Zhongbao Yoo, In-Kwon Yoon, Jongik Yu, Weilin Yuan, Xianbao Yushmanov, Igor Zach, Cenek Zampolli, Chiara Zaporozhets, Sergey Zarochentsev, Andrey Zavada, Petr Zaviyalov, Nikolai Zbroszczyk, Hanna Paulina Zelnicek, Pierre Zgura, Sorin Ion Zhalov, Mikhail Zhang, Xiaoming Zhang, Haitao Zhou, Fengchu Zhou, Daicui Zhou, You Zhu, Jianhui Zhu, Jianlin Zhu, Xiangrong Zichichi, Antonino Zimmermann, Alice Zinovjev, Gennady Zoccarato, Yannick Denis Zynovyev, Mykhaylo Zyzakbz, Maksym CA ALICE Collaboration TI Measurement of prompt J/psi and beauty hadron production cross sections at mid-rapidity in pp collisions at root s=7 TeV SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron Scattering ID QED RADIATIVE-CORRECTIONS; UNIVERSAL MONTE-CARLO; P(P)OVER-BAR COLLISIONS; QUARK PRODUCTION; DECAYS; PHOTOS AB The ALICE experiment at the LHC has studied J/psi production at mid-rapidity in pp collisions at root s = 7 TeV through its electron pair decay on a data sample corresponding to an integrated luminosity L-int = 5.6 nb(-1). The fraction of J/psi from the decay of long-lived beauty hadrons was determined for J/psi candidates with transverse momentum p(t) > 1,3 GeV/c and rapidity vertical bar y vertical bar < 0.9. The cross section for prompt J/psi mesons, i.e. directly produced J/psi and prompt decays of heavier charmonium states such as the psi(2S) and chi(c) resonances, is sigma(prompt J/psi) (p(t) > 1.3 GeV/c, vertical bar y vertical bar < 0.9) = 8.3 +/- 0.8(stat.) +/- 1.1 (syst.)(-1.4)(+1.5) (syst. pol.) mu b. The cross section for the production of b-hadrons decaying to J/psi with p(t) > 1.3 GeV/c and vertical bar y vertical bar < 0.9 is a sigma(J/psi <- hB) (p(t) > 1.3 GeV/c, vertical bar y vertical bar < 0.9) = 1.46 +/- 0.38 (stat.)(-0.32)(+0.26) (syst.) mu b. The results are compared to QCD model predictions. 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[Alici, Andrea; Ferroli, Rinaldo Baldini; Cifarelli, Luisa; Coccetti, Fabrizio; De Caro, Annalisa; Noferini, Francesco; Preghenella, Roberto; Santoro, Romualdo; Zichichi, Antonino] Ctr Studi & Ric, Ctr Fermi, Rome, Italy. [Alici, Andrea; Ferroli, Rinaldo Baldini; Cifarelli, Luisa; Coccetti, Fabrizio; De Caro, Annalisa; Noferini, Francesco; Preghenella, Roberto; Santoro, Romualdo; Zichichi, Antonino] Museo Stor Fis Enrico Fermi, Rome, Italy. [Garcia-Solis, Edmundo] Chicago State Univ, Chicago, IL USA. [Baldisseri, Alberto; Borel, Herve; Castellanos, Javier Ernesto Castillo; Charvet, Jean-Luc Fernand; Geuna, Claudio; Pal, S.; Da Costa, Hugo Denis Antonio Pereira; Rakotozafindrabe, Andry Malala; Yang, Hongyan] IRFU, Commissariat Energie Atom, Saclay, France. [Armesto, Nestor; Gonzalez Ferreiro, Elena; Pajares, Carlos; Albert Salgado, Carlos] Univ Santiago de Compostela, Dept Fis Particulas, Santiago De Compostela, Spain. [Armesto, Nestor; Gonzalez Ferreiro, Elena; Pajares, Carlos; Albert Salgado, Carlos] Univ Santiago de Compostela, IGFAE, Santiago De Compostela, Spain. [Ahmad, Arshad; Ahmad, Nazeer; Azmi, Mohd Danish; Irfan, Muhammad; Khan, Mohisin Mohammed] Aligarh Muslim Univ, Dept Phys, Aligarh 202002, Uttar Pradesh, India. [Altinpinar, Sedat; Djuvsland, Oeystein; Fehlker, Dominik; Haaland, Oystein Senneset; Huang, Meidana; Kanaki, Kalliopi; Langoy, Rune; Lien, Jorgen; Liu, Lijiao; Loenne, Per-Ivar; Nystrand, Joakim Ingemar; Roed, Ketil; Rohrich, Dieter; Skjerdal, Kyrre; Szostak, Artur Krzysztof; Ullaland, Kjetil; Vrebekk, Gaute; Wagner, Boris; Yang, Shiming] Univ Bergen, Dept Phys & Technol, Bergen, Norway. [Anson, Christopher Daniel; Bock, Nicolas; Gangadharan, Dhevan Raja; Humanic, Thomas; Lisa, Michael Annan; Salzwedel, Jai; Steinpreis, Matthew; Truesdale, David Christopher] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. 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[Bianchin, Chiara; Caffarri, Davide; Dainese, Andrea; Fabris, Daniela; Lunardon, Marcello; Morando, Maurizio; Moretto, Sandra; Rossi, Andrea; Scarlassara, Fernando; Segato, Gianfranco; Soramel, Francesca; Viesti, Giuseppe] Univ Padua, Dipartimento Fis, Padua, Italy. [Antinori, Federico; Bianchin, Chiara; Caffarri, Davide; Dainese, Andrea; Fabris, Daniela; Lunardon, Marcello; Morando, Maurizio; Moretto, Sandra; Rossi, Andrea; Scarlassara, Fernando; Segato, Gianfranco; Soramel, Francesca; Turrisi, Rosario; Viesti, Giuseppe] Sezione Ist Nazl Fis Nucl, Padua, Italy. [Camerini, Paolo; Contin, Giacomo; Lea, Ramona; Margagliotti, Giacomo Vito; Rui, Rinaldo; Venaruzzo, Massimo] Univ Trieste, Dipartimento Fis, Trieste, Italy. [Camerini, Paolo; Contin, Giacomo; Fragiacomo, Enrico; Grion, Nevio; Lea, Ramona; Margagliotti, Giacomo Vito; Piano, Stefano; Rachevski, Alexandre; Rui, Rinaldo; Venaruzzo, Massimo] Sezione Ist Nazl Fis Nucl, Trieste, Italy. [Agostinelli, Andrea; Arcelli, Silvia] Univ Bologna, Dipartimento Fis, Bologna, Italy. [Agostinelli, Andrea; Alici, Andrea; Antonioli, Pietro; Arcelli, Silvia; Romeo, Giovanni Cara; Cindolo, Federico; Hatzifotiadou, Despoina; Margotti, Anselmo; Nania, Rosario; Noferini, Francesco; Pesci, Alessandro; Preghenella, Roberto; Williams, Crispin; Zampolli, Chiara] Sezione Ist Nazl Fis Nucl, Bologna, Italy. [Basile, Maurizio; Bellini, Francesca; Cifarelli, Luisa; Falchieri, Davide; Guerzoni, Barbara; Meddi, Franco; Scioli, Gilda; Zichichi, Antonino] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Basile, Maurizio; Bellini, Francesca; Cifarelli, Luisa; Di Liberto, Sergio; Falchieri, Davide; Guerzoni, Barbara; Mazzoni, Alessandra Maria; Meddi, Franco; Scioli, Gilda; Urciuoli, Guido Marie; Zichichi, Antonino] Sezione Ist Nazl Fis Nucl, Rome, Italy. [Barbera, Roberto; La Rocca, Paola; Petta, Catia; Pulvirenti, Alberto; Riggi, Francesco] Univ Catania, Dipartimento Fis & Astron, Catania, Italy. [Barbera, Roberto; La Rocca, Paola; Palmeri, Armando; Pappalardo, Giuseppe; Petta, Catia; Pulvirenti, Alberto; Riggi, Francesco] Sezione Ist Nazl Fis Nucl, Catania, Italy. [De Caro, Annalisa; De Gruttola, Daniele; De Pasquale, Salvatore; Girard, Mario Fusco; Pagano, Paola; Virgili, Tiziano] Univ Salerno, Dipartimento Fis ER Caianiello, I-84100 Salerno, Italy. [De Caro, Annalisa; De Gruttola, Daniele; De Pasquale, Salvatore; Girard, Mario Fusco; Pagano, Paola; Virgili, Tiziano] Grp Collegato INFN, Salerno, Italy. [Beole, Stefania; Bianchi, Livio; Bossu, Francesco; Bruna, Elena; Bufalino, Stefania; Morales, Yasser Corrales; Ferretti, Alessandro; Gagliardi, Martino; Gallio, Mauro; Innocenti, Gian Michele; Marchisone, Massimiliano; Masera, Massimo; Milano, Leonardo; Ortona, Giacomo; Padilla, Fatima; Poghosyan, Martin; Siciliano, Melinda; Vasquez, Martin Alfonso Subieta; Vercellin, Ermanno] Univ Turin, Dipartimento Fis Sperimentale, Turin, Italy. [Alessandro, Bruno; Arnaldi, Roberta; Bala, Renu; Beole, Stefania; Berzano, Dario; Bianchi, Livio; Bossu, Francesco; Bruna, Elena; Bufalino, Stefania; Cerello, Piergiorgio; Morales, Yasser Corrales; De Marco, Nora; Ferretti, Alessandro; Gagliardi, Martino; Gallio, Mauro; Innocenti, Gian Michele; Leoncino, Marco; Manceau, Loic Henri Antoine; Marchisone, Massimiliano; Masera, Massimo; Milano, Leonardo; Monteno, Marco; Musso, Alfredo; Oppedisano, Chiara; Ortona, Giacomo; Padilla, Fatima; Piccotti, Anna; Poghosyan, Martin; Prino, Francesco; Riccati, Lodovico; Scomparin, Enrico; Siciliano, Melinda; Vasquez, Martin Alfonso Subieta; Toscano, Luca; Vercellin, Ermanno] Sezione Ist Nazl Fis Nucl, Turin, Italy. [Cortese, Pietro; Ferretti, Roberta; Ramello, Luciano; Senyukov, Serhiy; Sitta, Mario] Univ Piemonte Orientale, Dipartimento Sci & Innovaz Tecnol, Alessandria, Italy. [Cortese, Pietro; Ferretti, Roberta; Ramello, Luciano; Senyukov, Serhiy; Sitta, Mario] Grp Collegato INFN, Alessandria, Italy. [Altini, Valerio; Barile, Francesco; Bruno, Giuseppe Eugenio; Colamaria, Fabio; Colella, Domenico; D'Erasmo, Ginevra; Di Bari, Domenico; Di Giglio, Carmelo; Fionda, Fiorella; Fiore, Enrichetta Maria; Ghidini, Bruno; Mastroserio, Annalisa; Nicassio, Maria; Perrino, Davide; Terrevoli, Cristina; Volpe, Giacomo] Dipartimento Interateneo Fis M Merlin, Bari, Italy. [Altini, Valerio; Barile, Francesco; Bruno, Giuseppe Eugenio; Colamaria, Fabio; Colella, Domenico; de Cataldo, Giacinto; D'Erasmo, Ginevra; Di Bari, Domenico; Di Giglio, Carmelo; Elia, Domenico; Fionda, Fiorella; Fiore, Enrichetta Maria; Ghidini, Bruno; Lenti, Vito; Manzari, Vito; Mastromarco, Mario; Mastroserio, Annalisa; Nappi, Eugenio; Nicassio, Maria; Paticchio, Vincenzo; Perrino, Davide; Terrevoli, Cristina; Volpe, Giacomo] Sezione Ist Nazl Fis Nucl, Bari, Italy. [Christiansen, Peter; Dobrin, Alexandru Florin; Gros, Philippe; Velasquez, Antonio Ortiz; Oskarsson, Anders Nils Erik; Richert, Tuva; Stenlund, Evert Anders] Lund Univ, Div Expt High Energy Phys, Lund, Sweden. [Rinella, Gianluca Aglieri; Augustinus, Andre; Pedrosa, Fernando Baltasar Dos Santos; Betev, Latchezar; Boccioli, Marco; Brun, Rene; Carena, Francesco; Carena, Wisla; Carminati, Federico; Montoya, Camilo Andres Carrillo; Cavicchioli, Costanza; Chapeland, Sylvain; Cheshkov, Cvetan; Barroso, Vasco Miguel Chibante; Chochula, Peter; Cifarelli, Luisa; del Valle, Zaida Conesa; Costa, Filippo; Di Mauro, Antonio; Divia, Roberto; Floris, Michele; Fuchs, Ulrich; Gheata, Andrei George; Gheata, Mihaela; Giubellino, Paolo; Grigoras, Costin; Grigoras, Alina Gabriela; Grosse-Oetringhaus, Jan Fiete; Grosso, Raffaele; Hayrapetyan, Arsen; Hristov, Peter Zahariev; Innocenti, Pier Giorgio; Jacholkowski, Adam Wlodzimierz; Jirden, Lennart; Uysal, Ayben Karasu; Kisiel, Adam Ryszard; Kluge, Alexander; Lechman, Mateusz; Leistam, Lars; Lippmann, Christian; Lohn, Stefan Bernhard; Luzzi, Cinzia; Mager, Magnus; Tobon, Cesar Augusto Marin; Martinengo, Paolo; Mastroserio, Annalisa; Miskowiec, Dariusz; Mohanty, Ajit Kumar; Molnar, Levente; Morsch, Andreas; Muller, Hans; Musa, Luciano; Niculescu, Mihai; Oeschler, Helmut Oskar; Perini, Diego; Peskov, Vladimir; Pinazza, Ombretta; Poghosyan, Martin; Pulvirenti, Alberto; Quercigh, Emanuele; Rademakers, Alphonse; Revol, Jean-Pierre; Riedler, Petra; Riegler, Werner; Rabacal, Bartolomeu Rodrigues Fernandes; Rossegger, Stefan; Rossi, Andrea; Safarik, Karel; Santoro, Romualdo; Schreiner, Steffen; Schukraft, Jurgen; Schutz, Yves Roland; Shahoyan, Ruben; Sicking, Eva; Simonetti, Giuseppe; Soos, Csaba; Tauro, Arturo; Telesca, Adriana; Toia, Alberica; Vyvre, Pierre Vande; Volpe, Giacomo; von Haller, Barthelemy; Wessels, Johannes] European Org Nucl Res CERN, Geneva, Switzerland. [Krawutschke, Tobias] Fachhsch Koln, Cologne, Germany. [Alme, Johan; Erdal, Hege Austrheim; Helstrup, Haavard; Hetland, Kristin Fanebust; Kileng, Bjarte] Bergen Univ Coll, Fac Engn, Bergen, Norway. [Broz, Michal; Janik, Rudolf; Meres, Michal; Pikna, Miroslav; Sitar, Branislav; Strmen, Peter; Szarka, Imrich] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Adam, Jaroslav; Bielcik, Jaroslav; Cepila, Jan; Krelina, Michal; Krus, Miroslav; Pachr, Milos; Petracek, Vojtech; Petran, Michal; Pospisil, Vladimir; Smakal, Radek; Tlusty, David; Vajzer, Michal; Wagner, Vladimir; Zach, Cenek] Czech Tech Univ, Fac Nucl Sci & Phys Engn, CR-16635 Prague, Czech Republic. [Bombara, Marek; Harmanova, Zuzana; Putis, Marian; Urban, Jozef; Vrlakova, Janka] Safarik Univ, Fac Sci, Kosice, Slovakia. [Alt, Torsten; Bach, Matthias Jakob; de Cuveland, Jan; Gerhard, Jochen; Gorbunov, Sergey; Kalcher, Sebastian; Kirsch, Stefan; Kisel, Ivan; Kretz, Matthias; Lindenstruth, Volker; Painke, Florian; Rettig, Felix Vincenz; Rohr, David; Steinbeck, Timm Morten; Toia, Alberica] Goethe Univ Frankfurt, Frankfurt Inst Adv Studies, Frankfurt, Germany. [Ahn, Sang Un; Baek, Yong Wook; Jung, Hyung Taik; Kim, Do Won; Kim, Mimae; Kim, Seon Hee; Kim, Jin Sook; Lee, Sung Chul; Lee, Ki Sang; Oh, Sun Kun] Gangneung Wonju Natl Univ, Kangnung, South Korea. [Aysto, Juha Heikki; Chang, Beomsu; Kalliokoski, Tuomo Esa Aukusti; Kim, Dong Jo; Kral, Jiri; Krizek, Filip; Loo, Kai Krister; Novitzky, Norbert; Raiha, Tomi Samuli; Rak, Jan; Rasanen, Sami Sakari; Sarkamo, Juho Jaako; Trzaska, Wladyslaw Henryk] Helsinki Inst Phys, Jyvaskyla, Finland. [Aysto, Juha Heikki; Chang, Beomsu; Kalliokoski, Tuomo Esa Aukusti; Kim, Dong Jo; Kral, Jiri; Krizek, Filip; Loo, Kai Krister; Novitzky, Norbert; Raiha, Tomi Samuli; Rak, Jan; Rasanen, Sami Sakari; Sarkamo, Juho Jaako; Trzaska, Wladyslaw Henryk] Univ Jyvaskyla, Jyvaskyla, Finland. [Sakaguchi, Hiroaki; Shigaki, Kenta; Sugitate, Toru] Hiroshima Univ, Hiroshima, Japan. [Cai, Xu; Luo, Jiebin; Ma, Ke; Mao, Yaxian; Wan, Renzhuo; Wang, Mengliang; Wang, Dong; Wang, Yaping; Yin, Zhongbao; Yuan, Xianbao; Zhang, Xiaoming; Zhang, Haitao; Zhou, Fengchu; Zhou, Daicui; Zhu, Jianhui; Zhu, Jianlin; Zhu, Xiangrong] Hua Zhong Normal Univ, Wuhan, Peoples R China. [Behera, Nirbhay Kumar; Dash, Sadhana; Jena, Satyajit; Meethaleveedu, Greeshma Koyithatta; Kumar, Jitendra; Nandi, Basanta Kumar; Nyatha, Anitha; Varma, Raghava] Indian Inst Technol, Bombay 400076, Maharashtra, India. [Sahoo, Raghunath] Indian Inst Technol, Indore, Madhya Pradesh, India. [Boyer, Bruno Alexandre; Das, Indranil; Espagnon, Bruno; Hadjidakis, Cynthia Marie; Hrivnacova, Ivana; Lakomov, Igor; Le Bornec, Yves; Suire, Christophe Pierre; Takaki, Daniel Jesus Tapia; Palomo, Lizardo Valencia] Univ Paris 11, CNRS, IPNO, IN2P3, F-91405 Orsay, France. [Bogolyubsky, Mikhail; Kharlov, Yury; Patalakha, Dmitri Ivanovich; Polichtchouk, Boris; Sadovsky, Sergey; Stolpovskiy, Mikhail] Inst High Energy Phys, Protvino, Russia. [Finogeev, Dmitry; Guberbr, Fedor; Karavichev, Oleg; Karavicheva, Tatiana; Karpechev, Evgeny; Konevskih, Artem; Kurepin, A. B.; Kurepin, A.; Maevskaya, Alla; Pshenichnov, Igor; Reshetin, Andrey] Acad Sci, Inst Nucl Res, Moscow, Russia. [Bjelogrlic, Sandro; Chojnacki, Marek; Christakoglou, Panagiotis; de Rooij, Raoul Stefan; Grelli, Alessandro; La Pointe, Sarah Louise; Luparello, Grazia; Mischke, Andre; Nooren, Gerardus; Peitzmann, Thomas; Reicher, Martijn; Snellings, Raimond; Thomas, Deepa; van Leeuwen, Marco; Veldhoen, Misha; Verweij, Marta; Zhou, You] Univ Utrecht, Natl Inst Subat Phys, Utrecht, Netherlands. [Bjelogrlic, Sandro; Chojnacki, Marek; Christakoglou, Panagiotis; de Rooij, Raoul Stefan; Grelli, Alessandro; La Pointe, Sarah Louise; Luparello, Grazia; Mischke, Andre; Nooren, Gerardus; Peitzmann, Thomas; Reicher, Martijn; Snellings, Raimond; Thomas, Deepa; van Leeuwen, Marco; Veldhoen, Misha; Verweij, Marta; Zhou, You] Univ Utrecht, Inst Subat Phys, Utrecht, Netherlands. [Akindinov, Alexander; Kaidalov, Alexei; Kiselev, Sergey; Mal'Kevich, Dmitry; Nedosekin, Alexander; Sultanov, Rishat; Voloshin, Kirill] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Krivda, Marian; Sandor, Ladislav; Vala, Martin] Slovak Acad Sci, Inst Expt Phys, Kosice 04353, Slovakia. [Ban, Jaroslav; Baral, Rama Chandra; Kalinak, Peter; Kralik, Ivan; Mahapatra, Durga Prasad; Pastircak, Blahoslav; Sahu, Pradip Kumar] Inst Phys, Bhubaneswar 751007, Orissa, India. [Mares, Jiri; Polak, Karel; Zavada, Petr] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Danu, Andrea; Felea, Daniel; Gheata, Mihaela; Haiduc, Maria; Hasegan, Dumitru; Mitu, Ciprian Mihai; Niculescu, Mihai; Sevcenco, Adrian; Stan, Ionel; Stan, Ionel; Zgura, Sorin Ion] Inst Space Sci, Bucharest, Romania. [Boettger, Stefan; Breitner, Timo Gunther; Engel, Heiko; Kebschull, Udo Wolfgang; Lara, Camilo Ernesto; Teixido, Jordi Pujol; Ulrich, Jochen; Zelnicek, Pierre] Goethe Univ Frankfurt, Inst Informat, Frankfurt, Germany. [Appelshauser, Harald; Arend, Andreas; Arslandok, Mesut; Bailhache, Raphaelle Marie; Baumann, Christoph Heinrich; Beck, Hans; Blume, Christoph; Book, Julian; Buesching, Henner; Hartig, Matthias; Heckel, Stefan Thomas; Kliemant, Michael; Kramer, Frederick; Kulakov, Igor; Kurepin, A.; Lehnert, Joerg Walter; Vargas, Hermes Leon; Luettig, Philipp; Pitz, Nora; Rascanu, Bogdan Theodor; Reichelt, Patrick; Renfordt, Rainer Arno Ernst; Schuchmann, Simone; Ulery, Jason Glyndwr; Yu, Weilin; Zyzakbz, Maksym] Goethe Univ Frankfurt, Inst Kernphys, D-6000 Frankfurt, Germany. [Kalweit, Alexander Philipp; Mager, Magnus; Oeschler, Helmut Oskar] Tech Univ Darmstadt, Inst Kernphys, Darmstadt, Germany. [Anielski, Jonas; Bathen, Bastian; Dietel, Thomas; Emschermann, David Philip; Feldkamp, Linus; Heide, Markus Ansgar; Klein-Bosing, Christian; Passfeld, Annika; Santo, Rainer; Wessels, Johannes; Westerhoff, Uwe; Wilde, Martin Rudolf; Wilk, Alexander] Univ Munster, Inst Kernphys, D-4400 Munster, Germany. [Cuautle, Eleazar; Dominguez, Isabel; Jimenez Bustamante, Raul Tonatiuh; Ladron de Guevara, Pedro; Maldonado Cervantes, Ivonne Alicia; Mayani, Daniel; Velasquez, Antonio Ortiz; Paic, Guy; Lezama, Edgar Perez; Peskov, Vladimir; Simatovic, Goran] Univ Nacl Autonoma Mexico, Inst Ciencias Nucl, Mexico City 04510, DF, Mexico. [Salazar, Saul Aguilar; Alfaro Molina, Jose Ruben; Almaraz Avina, Erick Jonathan; Belmont-Moreno, Ernesto; Cruz Alaniz, Emilia; Helena Gonzalez-Trueba, Laura; Grabski, Varlen; Leon, Hermes; Davalos, Arnulfo Martinez; Alejandro Menchaca-Rocha, Arturo; Sandoval, Andres; Serradilla, Eulogio] Univ Nacl Autonoma Mexico, Inst Fis, Mexico City 01000, DF, Mexico. [Redlich, Krzysztof] Univ Wroclaw, Inst Theoret Phys, PL-50138 Wroclaw, Poland. [Belikov, Iouri; Hippolyte, Boris; Jangal, Swensy Gwladys; Kuhn, Christian Claude; Roy, Christelle Sophie; Castro, Xitzel Sanchez; Senyukov, Serhiy; Wan, Renzhuo] Univ Strasbourg, CNRS, IPHC, IN2P3, Strasbourg, France. [Batyunya, Boris; Fedunov, Anatoly; Grigoryan, Smbat; Nomokonov, Petr; Pocheptsov, Timur; Shabratova, Galina; Vala, Martin; Vodopianov, Alexander; Zaporozhets, Sergey] Joint Inst Nucl Res, Dubna, Russia. [Agocs, Andras Cabor; Barnafoldi, Gergely Gabor; Bencedi, Gyula; Berenyi, Daniel; Boldizsar, Laszlo; Denes, Ervin; Hamar, Gergoe; Levai, Peter; Pochybova, Sona] Hungarian Acad Sci, KFKI Res Inst Particle & Nucl Phys, Budapest, Hungary. [Tsuji, Tomoya; Ulrich, Jochen] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Ahn, Sul-Ah; Jang, Haeng Jin] Korea Inst Sci & Technol Informat, Taejon, South Korea. [Ahn, Sang Un; Baek, Yong Wook; Baldit, Alain; Barret, Valerie; Bastid, Nicole; Crochet, Philippe; Dupieux, Pascal; Ichou, Raphaelle; Lopez, Xavier Bernard; Manso, Franck; Marchisone, Massimiliano; Porteboeuf-Houssais, Sarah; Rosnet, Philippe; Vulpescu, Bogdan; Zhang, Xiaoming] Univ Clermont Ferrand, Clermont Univ, CNRS, LPC,IN2P3, Clermont Ferrand, France. [Arbor, Nicolas; Balbastre, Gustavo Conesa; Faivre, Julien; Furget, Christophe; Guernane, Rachid; Kox, Serge; Real, Jean-Sebastien; Silvestre, Catherine] Univ Grenoble 1, CNRS, Inst Polytech Grenoble, LPSC,IN2P3, Grenoble, France. [Bianchi, Nicola; Diaz, Amaya Ofelia Casanova; Cunqueiro, Leticia; Di Nezza, Pasquale; Fantoni, Alessandra; Gianotti, Paola; Muccifora, Valeria; Reolon, Anna Rita; Ronchetti, Federico] Ist Nazl Fis Nucl, Lab Nazl Frascati, I-00044 Frascati, Italy. [Ricci, Renato Angelo; Vannucci, Luigi] Ist Nazl Fis Nucl, Lab Nazl Legnaro, I-35020 Legnaro, Italy. [Braidot, Ermes; Cosentino, Mauro Rogerio; Fenton-Olsen, Bo; Jacobs, Peter; Loizides, Constantinos; Ploskon, Mateusz Andrzej; Sakai, Shingo] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Bogdanov, Alexey; Grigoriev, Vladislav; Kaplin, Vladimir; Kondratyeva, Natalia; Loginov, Vitaly; Malinina, Ludmila] Moscow Engn Phys Inst, Moscow 115409, Russia. [Andrei, Cristian; Berceanu, Ionela; Bercuci, Alexandru; Catanescu, Vasile; Herghelegiu, Andrei Ionut; Petris, Mariana; Petrovici, Mihai; Pop, Amalia; Schiaua, Claudiu Cornel] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Bilandzic, Ante; Boggild, Hans; Christensen, Christian Holm; Dalsgaard, Hans Hjersing; Gaardhoje, Jens Joergen; Gulbrandsen, Kristjan Herlache; Hansen, Alexander; Nielsen, Borge Svane; Nygaard, Casper; Sogaard, Carsten] Univ Copenhagen, Niels Bohr Inst, DK-2100 Copenhagen, Denmark. [Bilandzic, Ante; Botje, Michiel; Christakoglou, Panagiotis; Kuijer, Paul; Lara, Carlos Eugenio Perez; Manso, Alis Rodriguez; van der Kolk, Naomi] Natl Inst Subat Phys, Amsterdam, Netherlands. [Adamova, Dagmar; Bielcikova, Jana; Kushpil, Vasily; Kushpil, Svetlana; Sumbera, Michal; Vajzer, Michal] Acad Sci Czech Republic, Inst Nucl Phys, Prague, Czech Republic. [Ganoti, Paraskevi; Silvermyr, David Olle Rickard] Oak Ridge Natl Lab, Oak Ridge, TN USA. [Berdnikov, Yaroslav; Ivanov, Vladimir; Khanzadeev, Alexei; Kryshen, Evgeny; Malaev, Mikhail; Nikulin, Vladimir; Samsonov, Vladimir; Zhalov, Mikhail] Petersburg Nucl Phys Inst, Gatchina, Russia. [Cherney, Michael Gerard; Nilsen, Bjorn Steven] Creighton Univ, Dept Phys, Omaha, NE 68178 USA. [Aggarwal, Madan; Bhati, Ashok Kumar; Chawla, Isha; Kurepin, A.; Rathee, Deepika; Sharma, Natasha] Panjab Univ, Dept Phys, Chandigarh 160014, India. [Spyropoulou-Stassinaki, Martha; Vasileiou, Maria] Univ Athens, Dept Phys, Athens, Greece. [Aphecetche, Laurent Bernard; Buthelezi, Edith Zinhle; Cleymans, Jean Willy Andre; Fearick, Roger Worsley; Foertsch, Siegfried Valentin; Steyn, Gideon Francois; Vilakazi, Zabulon] Univ Cape Town, Dept Phys, IThemba LABS, ZA-7925 Cape Town, South Africa. [Bhasin, Anju; Gupta, Anik; Gupta, Ramni; Mangotra, Lalit Kumar; Potukuchi, Baba; Sambyal, Sanjeev Singh; Sharma, Satish; Sharma, Rohini; Singh, Ranbir] Univ Jammu, Dept Phys, Jammu 180004, India. [Goswami, Ankita; Mishra, Aditya Nath; Raniwala, Sudhir; Raniwala, Rashmi] Univ Rajasthan, Dept Phys, Jaipur 302004, Rajasthan, India. [Anguelov, Venelin; Busch, Oliver; Constantin, Paul; Glassel, Peter; Grajcarek, Robert; Herrmann, Norbert; Klein, Jochen; Koch, Kathrin; Krawutschke, Tobias; Kweon, Min Jung; Lohner, Daniel; Lu, Xianguo; Maire, Antonin; Perez, Jorge Mercado; Oyama, Ken; Pachmayer, Yvonne Chiara; Radomski, Sylwester; Reygers, Klaus Johannes; Schicker, Rainer Martin; Schweda, Kai Oliver; Stachel, Johanna; Stiller, Johannes Hendrik; Vallero, Sara; Wang, Yifei; Windelband, Bernd Stefan; Zimmermann, Alice] Heidelberg Univ, Inst Phys, D-6900 Heidelberg, Germany. [Browning, Tyler Allen; Scharenberg, Rolf Paul; Srivastava, Brijesh Kumar] Purdue Univ, W Lafayette, IN 47907 USA. [Chung, Suh-Urk; Song, Jihye; Yi, JunGyu; Yoo, In-Kwon] Pusan Natl Univ, Pusan 609735, South Korea. [Andronic, Anton; Arsene, Ionut Cristian; Averbeck, Ralf Peter; Braun-Munzinger, Peter; Hernandez, Juan Francisco Castillo; Donigus, Benjamin; Fasel, Markus; Foka, Panagiota; Frankenfeld, Ulrich Michael; Garabatos, Jose; Gonschior, Alexey; Gutbrod, Hans; Ivan, Cristian George; Ivanov, Marian; Knichel, Michael Linus; Kohler, Markus; Kraus, Ingrid Christine; Krzewicki, Mikolaj; Kurepin, A. B.; Kurepin, A.; Lippmann, Christian; Malzacher, Peter; Marin, Ana Maria; Masciocchi, Silvia; Miskowiec, Dariusz; Otwinowski, Jacek Tomasz; Park, Woo Jin; Romita, Rosa; Schmidt, Christian Joachim; Schwarz, Kilian Eberhard; Schweda, Kai Oliver; Selioujenkov, Ilya; Thader, Jochen Mathias; Vranic, Danilo] GSI Helmholtzzentrum Schwerionenforsch, Div Res, Darmstadt, Germany. [Andronic, Anton; Arsene, Ionut Cristian; Averbeck, Ralf Peter; Braun-Munzinger, Peter; Hernandez, Juan Francisco Castillo; Donigus, Benjamin; Fasel, Markus; Foka, Panagiota; Frankenfeld, Ulrich Michael; Garabatos, Jose; Gonschior, Alexey; Gutbrod, Hans; Ivan, Cristian George; Ivanov, Marian; Knichel, Michael Linus; Kohler, Markus; Kraus, Ingrid Christine; Krzewicki, Mikolaj; Lippmann, Christian; Malzacher, Peter; Marin, Ana Maria; Masciocchi, Silvia; Miskowiec, Dariusz; Otwinowski, Jacek Tomasz; Park, Woo Jin; Romita, Rosa; Schmidt, Christian Joachim; Schwarz, Kilian Eberhard; Schweda, Kai Oliver; Selioujenkov, Ilya; Thader, Jochen Mathias; Vranic, Danilo] GSI Helmholtzzentrum Schwerionenforsch, ExtreMe Matter Inst EMMI, Darmstadt, Germany. [Anticic, Tome; Nikolic, Vedran; Simatovic, Goran; Susa, Tatjana] Rudjer Boskovic Inst, Zagreb, Croatia. [Budnikov, Dmitry; Demanov, Vyacheslav; Filchagin, Sergey; Ilkaev, Radiy; Korneev, Andrey; Kuryakin, Alexey; Mamonov, Alexander; Naumov, Nikolay; Nazarenko, Sergey; Nazarov, Gleb; Puchagin, Sergey; Punin, Valery; Strabykin, Kirill; Sukhorukov, Mikhail; Tumkin, Alexandr; Vikhlyantsev, Oleg; Vinogradov, Yury; Vyushin, Alexey; Zaviyalov, Nikolai] Russian Fed Nucl Ctr VNIIEF, Sarov, Russia. [Aleksandrov, Dmitry; Blau, Dmitry; Fokin, Sergey; Ippolitov, Mikhail; Kazantsev, Andrey; Kucheriaev, Yury; Manko, Vladislav; Nikolaev, Sergey; Nikulin, Sergey; Nyanin, Alexandre; Peresunko, Dmitri; Ryabinkin, Evgeny; Sibiriak, Yury; Vasiliev, Andrey; Vinogradov, Alexander; Yasnopolsky, Stanislav; Yushmanov, Igor] Russian Res Ctr Kurchatov Inst, Moscow, Russia. [Bose, Suvendu Nath; Chattopadhyay, Sukalyan; Das, Debasish; Das, Kushal; Majumdar, A. K. Dutta; Khan, Palash; Roy, Pradip Kumar; Sinha, Tinku] Saha Inst Nucl Phys, Kolkata, India. [Barnby, Lee Stuart; Evans, David; Hanratty, Luke David; Jones, Peter Graham; Jusko, Anton; Kour, Ravjeet; Krivda, Marian; Lazzeroni, Cristina; Lee, Graham Richard; Lietava, Roman; Matthews, Zoe Louise; Navin, Sparsh; Palaha, Arvinder Singh; Petrov, Plamen Rumenov; Santoro, Romualdo; Scott, Patrick Aaron; Baillie, Orlando Villalobos] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Calvo Villar, Ernesto; Gago, Alberto; Guerra Gutierrez, Cesar] Pontificia Univ Catolica Peru, Dept Ciencias, Secc Fis, Lima, Peru. [Badala, Angela; Deloff, Andrzej; Dobrowolski, Tadeusz Antoni; Ilkiv, Iryna; Kurashvili, Podist; Redlich, Krzysztof; Riggi, Francesco; Siemiarczuk, Teodor; Stefanek, Grzegorz; Wilk, Grzegorz Andrzej] Soltan Inst Nucl Studies, PL-00681 Warsaw, Poland. [Batigne, Guillaume; Bergognon, Anais Annick Erica; Bregant, Marco; Delagrange, Hugues; Driga, Olga; Estienne, Magali Danielle; Germain, Marie; Lardeux, Antoine Xavier; Lefevre, Frederic; Lenhardt, Matthieu Laurent; Luquin, Lionel; Garcia, Gines Martinez; Mas, Alexis Jean-Michel; Massacrier, Laure Marie; Matyja, Adam Tomasz; Pillot, Philippe; Schutz, Yves Roland; Shabetai, Alexandre; Stocco, Diego] Univ Nantes, Ecole Mines Nantes, CNRS, SUBATECH,IN2P3, Nantes, France. [Gotovac, Sven; Mudnic, Eugen; Vickovic, Linda] Tech Univ Split FESB, Split, Croatia. [Bartke, Jerzy Gustaw; Figiel, Jan; Gladysz-Dziadus, Ewa; Kowalski, Marek; Matyja, Adam Tomasz; Mayer, Christoph; Rybicki, Andrzej; Sputowska, Iwona; Szczepankiewicz, Adam] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Knospe, Anders Garritt; Markert, Christina; Karampatsos, Leonidas Xaplanteris] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Gomez, Ramon; Leon Monzon, Ildefonso; Podesta Lerma, Pedro Luis Manuel] Univ Autonoma Sinaloa, Culiacan, Mexico. [Carlin Filho, Nelson; de Barros, Gabriel; Deppman, Airton; Figueredo, Marcel; Moreira De Godoy, Denise Aparecida; Munhoz, Marcelo; De Oliveira Filho, Elienos Pereira; do Passo Suaide, Alexandre Alarcon; de Toledo, Alejandro Szanto] Univ Sao Paulo, Sao Paulo, Brazil. [Chinellato, David; Dash, Ajay Kumar; Takahashi, Jun] Univ Estadual Campinas UNICAMP, Campinas, SP, Brazil. [Cheshkov, Cvetan; Cheynis, Brigitte; Ducroux, Laurent; Grossiord, Jean-Yves; Guilbaud, Maxime Rene Joseph; Massacrier, Laure Marie; Tieulent, Raphael Noel; Uras, Antonio; Zoccarato, Yannick Denis] Univ Lyon 1, CNRS, IPN Lyon, IN2P3, F-69622 Villeurbanne, France. [Bellwied, Rene; Blanco, Francesco; Jayarathna, Sandun; Madagodahettige-Don, Dilan Minthaka; Pinsky, Lawrence; Piyarathna, Danthasinghe; Seo, Jeewon; Timmins, Anthony; Weber, Michael] Univ Houston, Houston, TX USA. Vienna Univ Technol, A-1040 Vienna, Austria. Austrian Acad Sci, A-1010 Vienna, Austria. [Martashvili, Irakli; Mazer, Joel; Nattrass, Christine; Read, Kenneth Francis; Scott, Rebecca] Univ Tennessee, Knoxville, TN USA. [Gunji, Taku; Hamagaki, Hideki; Hori, Yasuto; Ozawa, Kyoichiro; Sano, Satoshi; Torii, Hisayuki; Yamaguchi, Yorito] Univ Tokyo, Tokyo, Japan. [Bhom, Jihyun; Chujo, Tatsuya; Esumi, Shinichi; Horaguchi, Takuma; Inaba, Motoi; Miake, Yasuo; Niida, Takafumi; Sakata, Dosatsu; Sano, Masato; Shimomura, Maya; Watanabe, Kengo] Univ Tsukuba, Tsukuba, Ibaraki, Japan. [Hess, Benjamin Andreas; Schmidt, Hans Rudolf; Wiechula, Jens] Univ Tubingen, Tubingen, Germany. [Ahammed, Zubayer; Basu, Sumit; Chattopadhyay, Subhasis; Choudhury, Subikash; De, Sudipan; Dubey, Anand Kumar; Majumdar, Mihir Ranjan Dutta; Ghosh, Premomoy; Khan, Shuaib Ahmad; Mohanty, Bedangadas; Muhuri, Sanjib; Mukherjee, Maitreyee; Nayak, Tapan Kumar; Pal, Susanta Kumar; Saini, Jogender; Singaraju, Rama Narayana; Singha, Subhash; Singhal, Vikas; Sinha, Bikash; Viyogi, Yogendra] Ctr Variable Energy Cyclotron, Kolkata, India. [Altsybeev, Igor; Asryan, Andzhey; Feofilov, Grigory; Ivanov, Andrey; Kolojvari, Anatoly; Kondratiev, Valery; Ochirov, Alexander; Vechernin, Vladimir; Vinogradov, Leonid; Zarochentsev, Andrey] St Petersburg State Univ, V Fock Inst Phys, St Petersburg, Russia. [Girard, Martin Robert; Graczykowski, Lukasz Kamil; Janik, Malgorzata Anna; Kisiel, Adam Ryszard; Oleniacz, Janusz; Ostrowski, Piotr Krystian; Pawlak, Tomasz Jan; Peryt, Wiktor Stanislaw; Pluta, Jan Marian; Szymanski, Maciej; Zbroszczyk, Hanna Paulina] Warsaw Univ Technol, Warsaw, Poland. [Borissov, Alexander; Cormier, Thomas Michael; Dobrin, Alexandru Florin; Jha, Deeptanshu Manu; Loggins, Vera; Mlynarz, Jocelyn; Pavlinov, Alexei; Prasad, Sidharth Kumar; Pruneau, Claude Andre; Putschke, Jorn Henning; Voloshin, Sergey; Yaldo, Chris G.] Wayne State Univ, Detroit, MI USA. [Adare, Andrew Marshall; Aronsson, Tomas Robert; Orduna, Diego Caballero; Caines, Helen Louise; Harris, John William; Hicks, Bernard; Hille, Per Thomas; Ma, Rongrong; Putschke, Jorn Henning; Smirnov, Nikolai] Yale Univ, New Haven, CT USA. [Grigoryan, Ara; Hayrapetyan, Arsen; Kakoyan, Vanik; Papikyan, Vardanush] Yerevan Phys Inst, Yerevan 375036, Armenia. [Uysal, Ayben Karasu] Yildiz Tekn Univ, Istanbul, Turkey. [Bearden, Ian Gardner; Chang, Beomsu; Kang, Ju Hwan; Kim, Minwoo; Kim, Beomkyu; Kim, Taesoo; Kwon, Youngil; Moon, Taebong; Scapparone, Eugenio; Song, Myunggeun; Yoon, Jongik] Yonsei Univ, Seoul 120749, South Korea. [Keidel, Ralf] Fachhsch Worms, ZTT, Worms, Germany. Moscow MV Lomonosov State Univ, DV Skohelt Inst Nucl Phys, Moscow, Russia. Univ Belgrade, Fac Phys, Belgrade, Serbia. Vinca Inst Nucl Sci, Belgrade, Serbia. RP Abelev, B (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RI Vickovic, Linda/F-3517-2017; HAMAGAKI, HIDEKI/G-4899-2014; Pshenichnov, Igor/A-4063-2008; Altsybeev, Igor/K-6687-2013; Janik, Malgorzata/O-7520-2015; Graczykowski, Lukasz/O-7522-2015; Adamova, Dagmar/G-9789-2014; Christensen, Christian/D-6461-2012; De Pasquale, Salvatore/B-9165-2008; de Cuveland, Jan/H-6454-2016; Kurepin, Alexey/H-4852-2013; Jena, Deepika/P-2873-2015; Yang, Hongyan/J-9826-2014; Turrisi, Rosario/H-4933-2012; Cosentino, Mauro/L-2418-2014; Bearden, Ian/M-4504-2014; Sumbera, Michal/O-7497-2014; Peitzmann, Thomas/K-2206-2012; Kharlov, Yuri/D-2700-2015; Mitu, Ciprian/E-6733-2011; Usai, Gianluca/E-9604-2015; Salgado, Carlos A./G-2168-2015; Bruna, Elena/C-4939-2014; Karasu Uysal, Ayben/K-3981-2015; Barnafoldi, Gergely Gabor/L-3486-2013; Christensen, Christian Holm/A-4901-2010; Chinellato, David/D-3092-2012; feofilov, grigory/A-2549-2013; Castillo Castellanos, Javier/G-8915-2013; Levai, Peter/A-1544-2014; Wagner, Vladimir/G-5650-2014; Vajzer, Michal/G-8469-2014; Krizek, Filip/G-8967-2014; Bielcikova, Jana/G-9342-2014; Blau, Dmitry/H-4523-2012; Jena, Satyajit/P-2409-2015; Akindinov, Alexander/J-2674-2016; Nattrass, Christine/J-6752-2016; Suaide, Alexandre/L-6239-2016; van der Kolk, Naomi/M-9423-2016; Deppman, Airton/J-5787-2014; Inst. of Physics, Gleb Wataghin/A-9780-2017; Ferreiro, Elena/C-3797-2017; Armesto, Nestor/C-4341-2017; Martinez Hernandez, Mario Ivan/F-4083-2010; Ferretti, Alessandro/F-4856-2013; Bregant, Marco/I-7663-2012; Vechernin, Vladimir/J-5832-2013; Zarochentsev, Andrey/J-6253-2013; Kondratiev, Valery/J-8574-2013; Felea, Daniel/C-1885-2012; Barnby, Lee/G-2135-2010; Barbera, Roberto/G-5805-2012; Sevcenco, Adrian/C-1832-2012; Takahashi, Jun/B-2946-2012; Mischke, Andre/D-3614-2011; Ramello, Luciano/F-9357-2013; Voloshin, Sergei/I-4122-2013 OI Vickovic, Linda/0000-0002-9820-7960; Pshenichnov, Igor/0000-0003-1752-4524; Altsybeev, Igor/0000-0002-8079-7026; Janik, Malgorzata/0000-0002-3356-3438; Christensen, Christian/0000-0002-1850-0121; De Pasquale, Salvatore/0000-0001-9236-0748; de Cuveland, Jan/0000-0003-0455-1398; Kurepin, Alexey/0000-0002-1851-4136; Jena, Deepika/0000-0003-2112-0311; Cosentino, Mauro/0000-0002-7880-8611; Bearden, Ian/0000-0003-2784-3094; Sumbera, Michal/0000-0002-0639-7323; Peitzmann, Thomas/0000-0002-7116-899X; Usai, Gianluca/0000-0002-8659-8378; Salgado, Carlos A./0000-0003-4586-2758; Bruna, Elena/0000-0001-5427-1461; Karasu Uysal, Ayben/0000-0001-6297-2532; Christensen, Christian Holm/0000-0002-1850-0121; Chinellato, David/0000-0002-9982-9577; feofilov, grigory/0000-0003-3700-8623; Castillo Castellanos, Javier/0000-0002-5187-2779; Jena, Satyajit/0000-0002-6220-6982; Akindinov, Alexander/0000-0002-7388-3022; Nattrass, Christine/0000-0002-8768-6468; Suaide, Alexandre/0000-0003-2847-6556; van der Kolk, Naomi/0000-0002-8670-0408; Deppman, Airton/0000-0001-9179-6363; Ferreiro, Elena/0000-0002-4449-2356; Armesto, Nestor/0000-0003-0940-0783; Martinez Hernandez, Mario Ivan/0000-0002-8503-3009; Ferretti, Alessandro/0000-0001-9084-5784; Vechernin, Vladimir/0000-0003-1458-8055; Zarochentsev, Andrey/0000-0002-3502-8084; Kondratiev, Valery/0000-0002-0031-0741; Felea, Daniel/0000-0002-3734-9439; Barnby, Lee/0000-0001-7357-9904; Barbera, Roberto/0000-0001-5971-6415; Sevcenco, Adrian/0000-0002-4151-1056; Takahashi, Jun/0000-0002-4091-1779; FU Calouste Gulbenkian Foundation from Lisbon and Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq); Financiadora de Estudos e Projetos (FINEP); Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC); Chinese Ministry of Education (CMOE); Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council; Carlsberg Foundation; Danish National Research Foundation; European Research Council under the European Community; Helsinki Institute of Physics; Academy of Finland French CNRS-IN2P3; 'Region Pays de Loire'; 'Region Alsace'; Region Auvergne'; CEA, France; German BMBF; Helmholtz Association; General Secretariat for Research and Technology, Ministry of Development, Greece; Hungarian OTKA; National Office for Research and Technology (NKTH); Department of Atomic Energy; Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN) of Italy; MEXT Grant-in-Aid for Specially Promoted Research Japan; Joint Institute for Nuclear Research, Dobna; National Research Foundation of Korea (NRF); CONACYT; DGAPA; Mexico; ALFA-EC; HELEN Program (High-Energy physics Latin-American European Network); Stichting voor Fundament eel Onderzoek der Materie (FOM); Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); Polish Ministry of Science and Higher Education; National Authority for Scientific Research - NASR (Autoritatea Natioala pentru Cercetare Stiintifica - ANCS); Federal Agency of Science of the Ministry of Education and Science of Russian Federation; International Science and Technology Center; Russian Academy of Sciences; Russian Federal Agency of Atomic Energy; Russian Federal Agency for Science and Innovations; CERN-INTAS; Ministry of Education of Slovakia; Department of Science and Technology, South Africa; CIEMAT; EELA; Ministerio de Educacion y Ciencia of Spain; Xunta de Galicia (Conselleria de Educacion); CEADEN; Cubaenergia; Cuba; IAEA (International Atomic Energy Agency); Swedish Research Council (VR); Knut & Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); United States Department of Energy; United States National Science Foundation; State of Texas; State of Ohio FX The ALICE collaboration acknowledges the following funding agencies for their support in building and running the ALICE detector:; Calouste Gulbenkian Foundation from Lisbon and Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq), Financiadora de Estudos e Projetos (FINEP), Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP);; National Natural Science Foundation of China (NSFC), the Chinese Ministry of Education (CMOE) and the Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council, the Carlsberg Foundation and the Danish National Research Foundation; The European Research Council under the European Community's Seventh Framework Programme; Helsinki Institute of Physics and the Academy of Finland French CNRS-IN2P3, the 'Region Pays de Loire', 'Region Alsace', Region Auvergne' and CEA, France;; German BMBF and the Helmholtz Association;; General Secretariat for Research and Technology, Ministry of Development, Greece;; Hungarian OTKA and National Office for Research and Technology (NKTH);; Department of Atomic Energy and Department of Science and Technology of the Government of India;; Istituto Nazionale di Fisica Nucleare (INFN) of Italy;; MEXT Grant-in-Aid for Specially Promoted Research Japan;; Joint Institute for Nuclear Research, Dobna;; National Research Foundation of Korea (NRF);; CONACYT, DGAPA, Mexico, ALFA-EC and the HELEN Program (High-Energy physics Latin-American European Network);; Stichting voor Fundament eel Onderzoek der Materie (FOM) and the Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands;; Research Council of Norway (NFR);; Polish Ministry of Science and Higher Education;; National Authority for Scientific Research - NASR (Autoritatea Natioala pentru Cercetare Stiintifica - ANCS);; Federal Agency of Science of the Ministry of Education and Science of Russian Federation, International Science and Technology Center, Russian Academy of Sciences, Russian Federal Agency of Atomic Energy, Russian Federal Agency for Science and Innovations and CERN-INTAS;; Ministry of Education of Slovakia;; Department of Science and Technology, South Africa;; CIEMAT, EELA, Ministerio de Educacion y Ciencia of Spain, Xunta de Galicia (Conselleria de Educacion), CEADEN, Cubaenergia, Cuba, and IAEA (International Atomic Energy Agency);; Swedish Research Council (VR) and Knut & Alice Wallenberg Foundation (KAW);; Ukraine Ministry of Education and Science;; United Kingdom Science and Technology Facilities Council (STFC);; The United States Department of Energy, the United States National Science Foundation, the State of Texas, and the State of Ohio. NR 48 TC 17 Z9 17 U1 1 U2 88 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD NOV PY 2012 IS 11 AR 065 DI 10.1007/JHEP11(2012)065 PG 31 WC Physics, Particles & Fields SC Physics GA 052KZ UT WOS:000312197800065 ER PT J AU Bodwin, GT Kim, UR Lee, J AF Bodwin, Geoffrey T. Kim, U-Rae Lee, Jungil TI Higher-order relativistic corrections to gluon fragmentation into spin-triplet S-wave quarkonium SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE NLO Computations; Hadronic Colliders ID ANTIQUARK BOUND-STATES; HEAVY QUARKONIUM; J/PSI PRODUCTION; J-PSI; ANNIHILATION; FACTORIZATION; TEVATRON; DECAY; NRQCD; LHC AB We compute the relative-order-nu(4) contribution to gluon fragmentation into quarkonium in the S-3(1) color-singlet channel, using the nonrelativistic QCD (NRQCD) factorization approach. The QCD fragmentation process contains infrared divergences that produce single and double poles in epsilon in 4 - 2 epsilon dimensions. We devise subtractions that isolate the pole contributions, which ultimately are absorbed into long-distance NRQCD matrix elements in the NRQCD matching procedure. The matching procedure involves two-loop renormalizations of the NRQCD operators. The subtractions are integrated over the phase space analytically in 4 -2 epsilon dimensions, and the remainder is integrated over the phase-space numerically. We find that the order-nu(4) contribution is enhanced relative to the order-nu(0) contribution. However, the order-nu(4) contribution is not important numerically at the current level of precision of quarkonium-hadroproduction phenomenology. We also estimate the contribution to hadroproduction from gluon fragmentation into quarkonium in the P-3(J) color-octet channel and find that it is significant in comparison to the complete next-to-leading-order-in-as contribution in that channel. C1 [Bodwin, Geoffrey T.] Argonne Natl Lab, HEP Div, Argonne, IL 60439 USA. [Kim, U-Rae; Lee, Jungil] Korea Univ, Dept Phys, Seoul 136713, South Korea. RP Bodwin, GT (reprint author), Argonne Natl Lab, HEP Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM gtb@hep.anl.gov; sadafada@korea.ac.kr; jungil@korea.ac.kr NR 51 TC 11 Z9 11 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD NOV PY 2012 IS 11 AR 020 DI 10.1007/JHEP11(2012)020 PG 40 WC Physics, Particles & Fields SC Physics GA 052KZ UT WOS:000312197800020 ER PT J AU Campbell, JM Giele, WT Williams, C AF Campbell, John M. Giele, Walter T. Williams, Ciaran TI The matrix element method at next-to-leading order SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE NLO Computations; Hadronic Colliders ID MODEL HIGGS-BOSON; JET CROSS-SECTIONS; ROOT-S=7 TEV; PP COLLISIONS; QUARK MASS; LHC; EVENTS; SEARCH AB This paper presents an extension of the matrix element method to next-to-leading order in perturbation theory, for electro-weak final states. TO accomplish this we have developed a method to calculate next-to-leading order weights on an event-by-event basis. This allows for the definition of next-to-leading order likelihoods in exactly the same fashion as at leading order, thus extending the matrix element method to next-to-leading order. A welcome by-product of the method is the straightforward and efficient generation of unweighted next-to-leading order events. As examples of the application of our next-to-leading order matrix element method we consider the measurement of the mass of the Z boson and also the search for the Higgs boson in the four lepton channel. C1 [Campbell, John M.; Giele, Walter T.; Williams, Ciaran] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. RP Campbell, JM (reprint author), Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. EM johnmc@fnal.gov; giele@fnal.gov; ciaran@fnal.gov FU United States Department of Energy [DE-AC02-07CH11359] FX We thank Oleg Brandt, Keith Ellis, Konstantin Matchev, Olivier Mattelaer and Gerben Stavenga for useful discussions. We thank Adam Martin for help with the Pythia sample generation. Fermilab is operated by Fermi Research Alliance, LLC under Contract No. DE-AC02-07CH11359 with the United States Department of Energy. NR 46 TC 21 Z9 21 U1 0 U2 4 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD NOV PY 2012 IS 11 AR 043 DI 10.1007/JHEP11(2012)043 PG 32 WC Physics, Particles & Fields SC Physics GA 052KZ UT WOS:000312197800043 ER PT J AU Sato, R Shirai, S Tobioka, K AF Sato, Ryosuke Shirai, Satoshi Tobioka, Kohsaku TI Gluino decay as a probe of high scale supersymmetry breaking SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Supersymmetry Phenomenology; Hadronic Colliders ID SPLIT SUPERSYMMETRY; STANDARD MODEL; ANOMALY MEDIATION; ROOT-S=7 TEV; BOSON MASS; LHC; SEARCH AB A supersymmetric standard model with heavier scalar supersymmetric particles has many attractive features. If the scalar mass scale is O(10 - 10(4)) TeV, the standard model like Higgs boson with mass around 125 GeV, which is strongly favored by the LHC experiment, can be realized. However, in this scenario the scalar particles are too heavy to be produced at the LHC. In addition, if the scalar mass is much less than O(10(4)) TeV, the lifetime of the gluino is too short to be measured. Therefore, it is hard to probe the scalar particles at a collider. However, a detailed study of the gluino decay reveals that two body decay of the gluino carries important information on the scalar scale. In this paper, we propose a test of this scenario by measuring the decay pattern of the gluino at the LHC. C1 [Sato, Ryosuke; Tobioka, Kohsaku] Univ Tokyo, Dept Phys, Tokyo 1130033, Japan. [Sato, Ryosuke; Tobioka, Kohsaku] Univ Tokyo, Todai Inst Adv Study, Kavli Inst Phys & Math Universe WPI, Kashiwa, Chiba 2778583, Japan. [Shirai, Satoshi] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Shirai, Satoshi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Theoret Phys Grp, Berkeley, CA 94720 USA. RP Sato, R (reprint author), Univ Tokyo, Dept Phys, Tokyo 1130033, Japan. EM rsato@hep-th.phys.s.u-tokyo.ac.jp; shirai@berkeley.edu; kohsaku.tobioka@ipmu.jp OI Sato, Ryosuke/0000-0003-2745-4208 FU JSPS; World Premier International Research Center Initiative (WPI Initiative), MEXT, Japan FX The work of RS and KT is supported in part by JSPS Research Fellowships for Young Scientists. This work is also supported by the World Premier International Research Center Initiative (WPI Initiative), MEXT, Japan. NR 57 TC 10 Z9 10 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD NOV PY 2012 IS 11 AR 041 DI 10.1007/JHEP11(2012)041 PG 23 WC Physics, Particles & Fields SC Physics GA 052KZ UT WOS:000312197800041 ER PT J AU Melnykov, V Chen, WC Maitra, R AF Melnykov, Volodymyr Chen, Wei-Chen Maitra, Ranjan TI MixSim: An R Package for Simulating Data to Study Performance of Clustering Algorithms SO JOURNAL OF STATISTICAL SOFTWARE LA English DT Article DE Gaussian mixture model; data simulation; pairwise overlap; parallel distribution plot; R ID 2 HIERARCHICAL CLUSTERINGS; SEPARATION AB The R package MixSim is a new tool that allows simulating mixtures of Gaussian distributions with different levels of overlap between mixture components. Pairwise overlap, defined as a sum of two misclassification probabilities, measures the degree of interaction between components and can be readily employed to control the clustering complexity of datasets simulated from mixtures. These datasets can then be used for systematic performance investigation of clustering and finite mixture modeling algorithms. Among other capabilities of MixSim, there are computing the exact overlap for Gaussian mixtures, simulating Gaussian and non-Gaussian data, simulating outliers and noise variables, calculating various measures of agreement between two partitionings, and constructing parallel distribution plots for the graphical display of finite mixture models. All features of the package are illustrated in great detail. The utility of the package is highlighted through a small comparison study of several popular clustering algorithms. C1 [Melnykov, Volodymyr] Univ Alabama, Dept Informat Syst Stat & Management Sci, Tuscaloosa, AL 35487 USA. [Chen, Wei-Chen] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. [Maitra, Ranjan] Iowa State Univ, Dept Stat & Stat Lab, Ames, IA 50011 USA. RP Melnykov, V (reprint author), Univ Alabama, Dept Informat Syst Stat & Management Sci, Tuscaloosa, AL 35487 USA. EM vmelnykov@ua.edu; wccsnow@gmail.com; maitra@iastate.edu RI Chen, Wei-Chen/G-4423-2013; OI Maitra, Ranjan/0000-0002-3515-8532 FU National Science Foundation CAREER Grant [DMS-0437555] FX The authors acknowledge partial support by the National Science Foundation CAREER Grant # DMS-0437555. We also thank the associate editor and reviewers whose comments and suggestions substantially improved the paper. NR 29 TC 26 Z9 26 U1 0 U2 11 PU JOURNAL STATISTICAL SOFTWARE PI LOS ANGELES PA UCLA DEPT STATISTICS, 8130 MATH SCIENCES BLDG, BOX 951554, LOS ANGELES, CA 90095-1554 USA SN 1548-7660 J9 J STAT SOFTW JI J. Stat. Softw. PD NOV PY 2012 VL 51 IS 12 BP 1 EP 25 PG 25 WC Computer Science, Interdisciplinary Applications; Statistics & Probability SC Computer Science; Mathematics GA 053RD UT WOS:000312289800001 ER PT J AU Semonin, OE Luther, JM Beard, MC AF Semonin, Octavi E. Luther, Joseph M. Beard, Matthew C. TI Quantum dots for next-generation photovoltaics SO MATERIALS TODAY LA English DT Review ID MULTIPLE EXCITON GENERATION; PBSE NANOCRYSTAL SOLIDS; JUNCTION SOLAR-CELLS; MULTIEXCITON GENERATION; COLLOIDAL NANOCRYSTALS; ELECTRICAL-PROPERTIES; CDSE NANOCRYSTALS; EFFICIENCY; FILMS; TRANSPORT AB Colloidal quantum-confined semiconductor nanostructures are an emerging class of functional material that are being developed for novel solar energy conversion strategies. One of the largest losses in a bulk or thin film solar cell occurs within a few picoseconds after the photon is absorbed, as photons with energy larger than the semiconductor bandgap produce charge-carriers with excess kinetic energy, which is then dissipated via phonon emission. Semiconductor nanostructures, where at least one dimension is small enough to produce quantum confinement effects, provide new pathways for controlling energy flow and therefore have the potential to increase the efficiency of the primary photoconversion step. In this review, we provide the current status of research efforts towards utilizing the unique properties of colloidal quantum dots (nanocrystals confined in three dimensions) in prototype solar cells and demonstrate that these unique systems have the potential to bypass the Shockley-Queisser single-junction limit for solar photon conversion. C1 [Semonin, Octavi E.; Luther, Joseph M.; Beard, Matthew C.] Natl Renewable Energy Lab, Chem & Mat Sci Ctr, Golden, CO 80401 USA. RP Beard, MC (reprint author), Natl Renewable Energy Lab, Chem & Mat Sci Ctr, Golden, CO 80401 USA. EM matt.beard@nrel.gov OI BEARD, MATTHEW/0000-0002-2711-1355 FU division of Chemical, Geoscience and Biosciences, within the office of Basic Energy Sciences, office of Science, US Department of Energy; Center for Advanced Solar Photophysics an Energy Frontier Research Center within the office of Basic Energy Sciences, Office of Sciences, US DOE; DOE [DE-AC36-086038308] FX We are thankful for the support of the division of Chemical, Geoscience and Biosciences, within the office of Basic Energy Sciences, office of Science, US Department of Energy for the work on the photophysics and chemistry of quantum dots. Our work on quantum dot solar cells was supported as part of the Center for Advanced Solar Photophysics an Energy Frontier Research Center within the office of Basic Energy Sciences, Office of Sciences, US DOE. Funding was provided to NREL under contract number DE-AC36-086038308 with DOE. NR 58 TC 59 Z9 61 U1 6 U2 276 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 1369-7021 J9 MATER TODAY JI Mater. Today PD NOV PY 2012 VL 15 IS 11 BP 508 EP 515 PG 8 WC Materials Science, Multidisciplinary SC Materials Science GA 052IN UT WOS:000312191300018 ER PT J AU Kohwi-Shigematsu, T Kohwi, Y Takahashi, K Richards, HW Ayers, SD Han, HJ Cai, ST AF Kohwi-Shigematsu, Terumi Kohwi, Yoshinori Takahashi, Keiko Richards, Hunter W. Ayers, Stephen D. Han, Hye-Jung Cai, Shutao TI SATB1-mediated functional packaging of chromatin into loops SO METHODS LA English DT Review DE Chromatin looping; Chromatin immunoprecipitation; SATB1; ChIP-3C; ChIP-4C ID MATRIX ATTACHMENT SEQUENCES; DNA-BINDING PROTEIN; IN-VIVO; CHROMOSOME CONFORMATION; GENE-EXPRESSION; GASTRIC-CANCER; NUCLEAR-MATRIX; SATB1; ORGANIZATION; SITES AB Mammalian genomes are organized into multiple layers of higher-order chromatin structure, and in this organization chromatin looping is a striking and crucial feature that brings together distal genomic loci into close spatial proximity. Such three-dimensional organization of chromatin has been suggested to be functionally important in gene regulation. Many important questions need to be addressed, such as what types of nuclear proteins are responsible for folding chromatin into loops, whether there are any genomic marks that serve as the core sites of chromatin folding events, how distal genomic sites are brought together, and what are the biological consequences for interactions between distal genomic loci. In order to address these fundamental questions, it is essential to devise and employ methods that can capture higher-order structures formed by specific nuclear proteins at high resolution. In this article, in order to describe methods of analyzing protein-mediated chromatin interactions, we will use as an example a global genome-organizer protein, SATB1, which mediates chromatin looping. Published by Elsevier Inc. C1 [Kohwi-Shigematsu, Terumi; Kohwi, Yoshinori; Takahashi, Keiko; Richards, Hunter W.; Han, Hye-Jung; Cai, Shutao] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. [Ayers, Stephen D.] Methodist Hosp, Res Inst, Houston, TX 77030 USA. RP Kohwi-Shigematsu, T (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. EM TKohwi-Shigematsu@lbl.gov RI Ayers, Stephen/O-4535-2014 OI Ayers, Stephen/0000-0003-1390-8969 FU National Cancer Institute [R37 CA39681]; Low Dose Radiation Research Program, US Department of Energy [DE-AC02-055CH11231] FX This project was supported by National Cancer Institute R37 CA39681 and Low Dose Radiation Research Program, US Department of Energy (DE-AC02-055CH11231). We thank Mr. Minyong Chung for helpful advise on the sequencing strategy. NR 51 TC 8 Z9 8 U1 0 U2 10 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 1046-2023 EI 1095-9130 J9 METHODS JI Methods PD NOV PY 2012 VL 58 IS 3 BP 243 EP 254 DI 10.1016/j.ymeth.2012.06.019 PG 12 WC Biochemical Research Methods; Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA 054RD UT WOS:000312360000007 PM 22782115 ER PT J AU Neumann, G Macken, CA Karasin, AI Fouchier, RAM Kawaoka, Y AF Neumann, Gabriele Macken, Catherine A. Karasin, Alexander I. Fouchier, Ron A. M. Kawaoka, Yoshihiro TI Egyptian H5N1 Influenza Viruses-Cause for Concern? SO PLOS PATHOGENS LA English DT Editorial Material ID RECEPTOR SPECIFICITY; HOST-RANGE; A VIRUSES; MIGRATORY WATERFOWL; TRANSMISSION; FERRETS; REPLICATION; POLYMERASE; EPITHELIUM; INFECTION C1 [Neumann, Gabriele; Karasin, Alexander I.; Kawaoka, Yoshihiro] Univ Wisconsin, Dept Pathobiol Sci, Madison, WI 53706 USA. [Macken, Catherine A.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM USA. [Fouchier, Ron A. M.] Erasmus MC, Dept Virol, Rotterdam, Netherlands. [Kawaoka, Yoshihiro] ERATO Infect Induced Host Responses Project, Saitama, Japan. [Kawaoka, Yoshihiro] Univ Tokyo, Inst Med Sci, Int Res Ctr Infect Dis, Dept Special Pathogens, Tokyo, Japan. [Kawaoka, Yoshihiro] Kobe Univ, Dept Microbiol & Infect Dis, Kobe, Hyogo, Japan. [Kawaoka, Yoshihiro] Univ Tokyo, Inst Med Sci, Div Virol, Dept Microbiol & Immunol, Tokyo, Japan. RP Neumann, G (reprint author), Univ Wisconsin, Dept Pathobiol Sci, Madison, WI 53706 USA. EM Kawaokay@svm.vetmed.wisc.edu RI Fouchier, Ron/A-1911-2014 OI Fouchier, Ron/0000-0001-8095-2869 FU PHS HHS [HHSN266200700010C] NR 27 TC 26 Z9 27 U1 0 U2 6 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1553-7374 J9 PLOS PATHOG JI PLoS Pathog. PD NOV PY 2012 VL 8 IS 11 AR e1002932 DI 10.1371/journal.ppat.1002932 PG 3 WC Microbiology; Parasitology; Virology SC Microbiology; Parasitology; Virology GA 049PY UT WOS:000311997100001 PM 23166487 ER PT J AU Aalseth, CE Bonicalzi, RM Cantaloub, MG Day, AR Erikson, LE Fast, J Forrester, JB Fuller, ES Glasgow, BD Greenwood, LR Hoppe, EW Hossbach, TW Hyronimus, BJ Keillor, ME Mace, EK McIntyre, JI Merriman, JH Myers, AW Overman, CT Overman, NR Panisko, ME Seifert, A Warren, GA Runkle, RC AF Aalseth, C. E. Bonicalzi, R. M. Cantaloub, M. G. Day, A. R. Erikson, L. E. Fast, J. Forrester, J. B. Fuller, E. S. Glasgow, B. D. Greenwood, L. R. Hoppe, E. W. Hossbach, T. W. Hyronimus, B. J. Keillor, M. E. Mace, E. K. McIntyre, J. I. Merriman, J. H. Myers, A. W. Overman, C. T. Overman, N. R. Panisko, M. E. Seifert, A. Warren, G. A. Runkle, R. C. TI A shallow underground laboratory for low-background radiation measurements and materials development SO REVIEW OF SCIENTIFIC INSTRUMENTS LA English DT Article ID COPPER; RADIOACTIVITY; RADIONUCLIDES; TECHNOLOGY; TREATY; AR-37 AB Pacific Northwest National Laboratory recently commissioned a new shallow underground laboratory, located at a depth of approximately 30 meters-water-equivalent. This new addition to the small class of radiation measurement laboratories located at modest underground depths houses the latest generation of custom-made, high-efficiency, low-background gamma-ray spectrometers and gas proportional counters. This paper describes the unique capabilities present in the shallow underground laboratory; these include large-scale ultra-pure materials production and a suite of radiation detection systems. Reported data characterize the degree of background reduction achieved through a combination of underground location, graded shielding, and rejection of cosmic-ray events. We conclude by presenting measurement targets and future opportunities. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4761923] C1 [Aalseth, C. E.; Bonicalzi, R. M.; Cantaloub, M. G.; Day, A. R.; Erikson, L. E.; Fast, J.; Forrester, J. B.; Fuller, E. S.; Glasgow, B. D.; Greenwood, L. R.; Hoppe, E. W.; Hossbach, T. W.; Hyronimus, B. J.; Keillor, M. E.; Mace, E. K.; McIntyre, J. I.; Merriman, J. H.; Myers, A. W.; Overman, C. T.; Overman, N. R.; Panisko, M. E.; Seifert, A.; Warren, G. A.; Runkle, R. C.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Aalseth, CE (reprint author), Pacific NW Natl Lab, POB 999, Richland, WA 99352 USA. RI McIntyre, Justin/P-1346-2014; Greenwood, Lawrence/H-9539-2016; OI McIntyre, Justin/0000-0002-3706-4310; Greenwood, Lawrence/0000-0001-6563-0650; Keillor, Martin/0000-0001-7828-5868; Day, Anthony/0000-0002-1217-1822 FU (U.S.) Department of Energy (DOE) by Battelle [DE-AC05-76RL01830] FX The authors thank Ned Wogman for his thorough review of this paper. This paper is PNNL Report no. SA-89084. Pacific Northwest National Laboratory is operated for the (U.S.) Department of Energy (DOE) by Battelle under Contract No. DE-AC05-76RL01830. NR 40 TC 17 Z9 17 U1 1 U2 19 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0034-6748 J9 REV SCI INSTRUM JI Rev. Sci. Instrum. PD NOV PY 2012 VL 83 IS 11 AR 113503 DI 10.1063/1.4761923 PG 10 WC Instruments & Instrumentation; Physics, Applied SC Instruments & Instrumentation; Physics GA 050DY UT WOS:000312034400015 PM 23206058 ER PT J AU Comstock, DJ Elam, JW Pellin, MJ Hersam, MC AF Comstock, David J. Elam, Jeffrey W. Pellin, Michael J. Hersam, Mark C. TI High aspect ratio nanoneedle probes with an integrated electrode at the tip apex SO REVIEW OF SCIENTIFIC INSTRUMENTS LA English DT Article ID ATOMIC-FORCE MICROSCOPY; GOLD NANOPARTICLE; FABRICATION; DEPOSITION; RESOLUTION; NANOELECTRODES; CANTILEVER; SILICON; GROWTH; SILVER AB Many nanoscale characterization techniques require high aspect ratio nanoneedle probes with an integrated electrode that is electrically insulated everywhere except at the tip apex. We report the utilization of electron beam induced deposition, focused ion beam milling, and atomic layer deposition to fabricate such probes at the sub-100 nm length scale. This fabrication method is highly reproducible and enables precise control of the probe dimensions. Subsequent electrodeposition at the integrated electrode enables customized functionalization of the tip apex. These probes have clear applications in scanning electrochemical microscopy-atomic force microscopy, magnetic force microscopy, apertureless near-field optical microscopy, and tip-enhanced Raman spectroscopy. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4767248] C1 [Comstock, David J.; Hersam, Mark C.] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. [Comstock, David J.; Elam, Jeffrey W.] Argonne Natl Lab, Div Energy Syst, Argonne, IL 60439 USA. [Pellin, Michael J.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Pellin, Michael J.; Hersam, Mark C.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. RP Comstock, DJ (reprint author), Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. EM m-hersam@northwestern.edu RI Pellin, Michael/B-5897-2008; Hersam, Mark/B-6739-2009 OI Pellin, Michael/0000-0002-8149-9768; FU Center for Electrical Energy Storage, an Energy Frontier Research Center; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; NSF-NSEC; NSF-MRSEC; Keck Foundation; State of Illinois; Northwestern University; NDSEG Fellowship; UChicago Argonne, LLC. [DE-AC02-06CH11357] FX This work was supported by the Center for Electrical Energy Storage, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences (DE-AC02-06CH11357). This research made use of public facilities within the NUANCE Center at Northwestern University. The NUANCE Center is supported by the NSF-NSEC, the NSF-MRSEC, the Keck Foundation, the State of Illinois, and the Northwestern University. D.J. Comstock further acknowledges support from an NDSEG Fellowship. Argonne National Laboratory (ANL) is a U. S. Department of Energy Office of Science Laboratory operated under contract (Contract No. DE-AC02-06CH11357) by UChicago Argonne, LLC. NR 30 TC 11 Z9 11 U1 2 U2 56 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0034-6748 J9 REV SCI INSTRUM JI Rev. Sci. Instrum. PD NOV PY 2012 VL 83 IS 11 AR 113704 DI 10.1063/1.4767248 PG 4 WC Instruments & Instrumentation; Physics, Applied SC Instruments & Instrumentation; Physics GA 050DY UT WOS:000312034400025 PM 23206068 ER PT J AU Dissanayake, DMNM Ashraf, A Pang, Y Eisaman, MD AF Dissanayake, D. M. N. M. Ashraf, A. Pang, Y. Eisaman, M. D. TI Guided-mode quantum efficiency: A novel optoelectronic characterization technique SO REVIEW OF SCIENTIFIC INSTRUMENTS LA English DT Article ID FILM SOLAR-CELLS; PHOTOVOLTAIC MATERIALS; WAVE-GUIDE; THIN-FILMS; DEVICES; LIMIT; ABSORPTION AB We demonstrate a novel, multi-purpose optoelectronic characterization technique to quantify light trapping and photoinduced charge generation and extraction in photovoltaics and other multilayer thin-film optoelectronic devices. The technique measures the photogenerated current created via the selective evanescent coupling of incident light into each of the guided modes of an optoelectronic device. In analogy to the internal quantum efficiency commonly used to characterize photovoltaics (the ratio of photogenerated electrons extracted from the device to photons absorbed by the device for normally incident light), we define the guided-mode internal quantum efficiency (GIQE) as the ratio of photogenerated electrons extracted from the device to the photons absorbed by the device for a specific guided mode. We complement the measurement of GIQE with computational modeling to calculate the electromagnetic field distribution within the various layers of the device, enabling us to separate the contribution to the GIQE of the absorption in the photoactive layer from parasitic absorption in other layers. By separately quantifying the quantum efficiency of each guided mode, this technique enables improved optimization and design of optoelectronic devices, including photovoltaics that utilize waveguiding and light-trapping. Additionally, since the electromagnetic field of each guided mode has a unique spatial distribution within the photoactive layer, this technique also provides insight into the spatial distributions of charge-carrier extraction, regions of disorder, trap states, and defects within the photoactive layer. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4768539] C1 [Dissanayake, D. M. N. M.; Ashraf, A.; Pang, Y.; Eisaman, M. D.] Brookhaven Natl Lab, Sustainable Energy Technol Dept, Upton, NY 11973 USA. [Ashraf, A.; Pang, Y.; Eisaman, M. D.] SUNY Stony Brook, Dept Phys, Stony Brook, NY 11794 USA. RP Eisaman, MD (reprint author), Brookhaven Natl Lab, Sustainable Energy Technol Dept, Upton, NY 11973 USA. EM meisaman@bnl.gov RI Eisaman, Matthew/E-8006-2011 OI Eisaman, Matthew/0000-0002-3814-6430 FU U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886]; U. S. Department of Energy, Sustainable Energy Technologies Department [DE-AC02-98CH10886] FX We thank J. Jackson and L. Steingart of Metricon Corp. for helpful discussions. At Brookhaven, we thank C.-Y. Nam, C. Black, D. Germack, D. Nykypanchuk, and M. Liu of the Center for Functional Nanomaterials for helpful discussions and equipment training. We also thank one anonymous reviewer for constructive suggestions. Research was carried out in part at the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. This work was also partially supported by the U. S. Department of Energy, Sustainable Energy Technologies Department under Contract No. DE-AC02-98CH10886. NR 34 TC 4 Z9 4 U1 0 U2 16 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0034-6748 J9 REV SCI INSTRUM JI Rev. Sci. Instrum. PD NOV PY 2012 VL 83 IS 11 AR 114704 DI 10.1063/1.4768539 PG 8 WC Instruments & Instrumentation; Physics, Applied SC Instruments & Instrumentation; Physics GA 050DY UT WOS:000312034400039 PM 23206082 ER PT J AU Honnicke, MG Manica, J Mazzaro, I Cusatis, C Huang, XR AF Hoennicke, M. G. Manica, J. Mazzaro, I. Cusatis, C. Huang, X. -R. TI Source effects in analyzer-based X-ray phase contrast imaging with conventional sources SO REVIEW OF SCIENTIFIC INSTRUMENTS LA English DT Article ID CUT CRYSTALS; RADIOGRAPHY; MONOCHROMATORS; MAMMOGRAPHY; TOMOGRAPHY; SCATTERING; ELETTRA; LNLS AB Several recent papers have shown the implementation of analyzer based X-ray phase contrast imaging (ABI) with conventional X-ray sources. The high flux is always a requirement to make the technique useful for bio-medical applications. Here, we present and discuss three important parameters, which need to be taken into account, when searching for the high flux ABI: anisotropic magnification, double image, and source size spread due to intrinsic dispersive diffraction by asymmetrically cut crystals. These parameters, if not well optimized, may cause important features in the acquired images which can mislead the interpretation. A few ways to minimize these effects are implemented and discussed, including some experimental results. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4767243] C1 [Hoennicke, M. G.] Univ Fed Integracao Latino Amer, BR-85867970 Foz Do Iguacu, PR, Brazil. [Manica, J.] Univ Estadual Oeste Parana, BR-85867970 Foz Do Iguacu, PR, Brazil. [Mazzaro, I.; Cusatis, C.] Univ Fed Parana, Dept Fis, LORXI, BR-81531990 Curitiba, PR, Brazil. [Huang, X. -R.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Honnicke, MG (reprint author), Univ Fed Integracao Latino Amer, BR-85867970 Foz Do Iguacu, PR, Brazil. EM marcelo.honnicke@unila.edu.br RI Cusatis, Cesar/N-7559-2014; Honnicke, Marcelo/I-8624-2012 OI Cusatis, Cesar/0000-0002-1621-3727; FU CNPq/PQ [305034/2010-3, 311570/2009-7]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX M. G. Honnicke is grateful to CNPq/PQ (305034/2010-3) for the financial support. C. Cusatis acknowledges CNPq/PQ (311570/2009-7) for his support. X.-R. Huang was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 30 TC 9 Z9 9 U1 0 U2 19 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0034-6748 J9 REV SCI INSTRUM JI Rev. Sci. Instrum. PD NOV PY 2012 VL 83 IS 11 AR 113702 DI 10.1063/1.4767243 PG 8 WC Instruments & Instrumentation; Physics, Applied SC Instruments & Instrumentation; Physics GA 050DY UT WOS:000312034400023 PM 23206066 ER PT J AU Reinke, ML Podpaly, YA Bitter, M Hutchinson, IH Rice, JE Delgado-Aparicio, L Gao, C Greenwald, M Hill, K Howard, T Hubbard, A Hughes, JW Pablant, N White, AE Wolfe, SM AF Reinke, M. L. Podpaly, Y. A. Bitter, M. Hutchinson, I. H. Rice, J. E. Delgado-Aparicio, L. Gao, C. Greenwald, M. Hill, K. Howard, T. Hubbard, A. Hughes, J. W. Pablant, N. White, A. E. Wolfe, S. M. TI X-ray imaging crystal spectroscopy for use in plasma transport research SO REVIEW OF SCIENTIFIC INSTRUMENTS LA English DT Article ID ALCATOR-C-MOD; ION TEMPERATURE; TOROIDAL PLASMA; TOKAMAK PLASMA; ROTATION; ENERGY; FIELD; JET AB This research describes advancements in the spectral analysis and error propagation techniques associated with x-ray imaging crystal spectroscopy (XICS) that have enabled this diagnostic to be used to accurately constrain particle, momentum, and heat transport studies in a tokamak for the first time. Doppler tomography techniques have been extended to include propagation of statistical uncertainty due to photon noise, the effect of non-uniform instrumental broadening as well as flux surface variations in impurity density. These methods have been deployed as a suite of modeling and analysis tools, written in interactive data language (IDL) and designed for general use on tokamaks. Its application to the Alcator C-Mod XICS is discussed, along with novel spectral and spatial calibration techniques. Example ion temperature and radial electric field profiles from recent I-mode plasmas are shown, and the impact of poloidally asymmetric impurity density and natural line broadening is discussed in the context of the planned ITER x-ray crystal spectrometer. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4758281] C1 [Reinke, M. L.; Podpaly, Y. A.; Hutchinson, I. H.; Rice, J. E.; Gao, C.; Greenwald, M.; Howard, T.; Hubbard, A.; Hughes, J. W.; White, A. E.; Wolfe, S. M.] MIT Plasma Sci & Fus Ctr, Cambridge, MA 02139 USA. [Bitter, M.; Delgado-Aparicio, L.; Hill, K.; Pablant, N.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. RP Reinke, ML (reprint author), MIT Plasma Sci & Fus Ctr, Cambridge, MA 02139 USA. RI Hutchinson, Ian/D-1136-2009; OI Hutchinson, Ian/0000-0003-4276-6576; Greenwald, Martin/0000-0002-4438-729X FU (U.S.) Department of Energy (DOE) [DE-FC02-99ER54512, DE-AC02-09CH11466] FX The authors would like to thank the engineering, technical and computing staff at the PSFC and PPPL for helping to make HIREXSR such a dramatic success. This work was supported by (U.S.) Department of Energy (DOE) contracts DE-FC02-99ER54512 and DE-AC02-09CH11466 and in part by an appointment to the DOE Fusion Energy Postdoctoral Research Program administered by ORISE. NR 38 TC 30 Z9 31 U1 0 U2 11 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0034-6748 J9 REV SCI INSTRUM JI Rev. Sci. Instrum. PD NOV PY 2012 VL 83 IS 11 AR 113504 DI 10.1063/1.4758281 PG 12 WC Instruments & Instrumentation; Physics, Applied SC Instruments & Instrumentation; Physics GA 050DY UT WOS:000312034400016 PM 23206059 ER PT J AU Rygg, JR Eggert, JH Lazicki, AE Coppari, F Hawreliak, JA Hicks, DG Smith, RF Sorce, CM Uphaus, TM Yaakobi, B Collins, GW AF Rygg, J. R. Eggert, J. H. Lazicki, A. E. Coppari, F. Hawreliak, J. A. Hicks, D. G. Smith, R. F. Sorce, C. M. Uphaus, T. M. Yaakobi, B. Collins, G. W. TI Powder diffraction from solids in the terapascal regime SO REVIEW OF SCIENTIFIC INSTRUMENTS LA English DT Article ID EQUATION-OF-STATE; COMPRESSION EXPERIMENTS; ISENTROPIC COMPRESSION; SHOCK COMPRESSION; PRESSURE; ALUMINUM; TANTALUM; METALS; KBAR AB A method of obtaining powder diffraction data on dynamically compressed solids has been implemented at the Jupiter and OMEGA laser facilities. Thin powdered samples are sandwiched between diamond plates and ramp compressed in the solid phase using a gradual increase in the drive-laser intensity. The pressure history in the sample is determined by back-propagation of the measured diamond free-surface velocity. A pulse of x rays is produced at the time of peak pressure by laser illumination of a thin Cu or Fe foil and collimated at the sample plane by a pinhole cut in a Ta substrate. The diffracted signal is recorded on x-ray sensitive material, with a typical d-spacing uncertainty of similar to 0.01 angstrom. This diagnostic has been used up to 0.9 TPa (9 Mbar) to verify the solidity, measure the density, constrain the crystal structure, and evaluate the strain-induced texturing of a variety of compressed samples spanning atomic numbers from 6 (carbon) to 82 (lead). Further refinement of the technique will soon enable diffraction measurements in solid samples at pressures exceeding 1 TPa. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4766464] C1 [Rygg, J. R.; Eggert, J. H.; Lazicki, A. E.; Coppari, F.; Hawreliak, J. A.; Hicks, D. G.; Smith, R. F.; Uphaus, T. M.; Collins, G. W.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Sorce, C. M.; Yaakobi, B.] Univ Rochester, Laser Energet Lab, Rochester, NY 14623 USA. RP Rygg, JR (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RI Hicks, Damien/B-5042-2015 OI Hicks, Damien/0000-0001-8322-9983 FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX The authors thank Stephanie Uhlich and Walt Unites for their valuable assistance in preparation of the PXRDIP targets, and to the operations staff at the Janus and OMEGA lasers who supported these experiments. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 40 TC 23 Z9 24 U1 3 U2 36 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0034-6748 J9 REV SCI INSTRUM JI Rev. Sci. Instrum. PD NOV PY 2012 VL 83 IS 11 AR 113904 DI 10.1063/1.4766464 PG 7 WC Instruments & Instrumentation; Physics, Applied SC Instruments & Instrumentation; Physics GA 050DY UT WOS:000312034400030 PM 23206073 ER PT J AU Sturtevant, BT Pantea, C Sinha, DN AF Sturtevant, Blake T. Pantea, Cristian Sinha, Dipen N. TI An acoustic resonance measurement cell for liquid property determinations up to 250 degrees C SO REVIEW OF SCIENTIFIC INSTRUMENTS LA English DT Article ID EQUATION-OF-STATE; PURE WATER; THERMODYNAMIC PROPERTIES; NONLINEARITY PARAMETER; ULTRASONIC-VELOCITY; SOUND VELOCITIES; PRESSURE; FLUIDS; SPEED; B/A AB This paper reports on the development of a compact, rugged, and portable measurement cell design for the determination of liquid sound speed at temperatures up to 250 degrees C and pressures up to 3000 psi. Although a significant amount of work exists in the literature on the characterization of fluids, primarily pure water, over a wide range of pressures and temperatures, the availability of experimentally determined sound speed in water between 100 degrees C and 250 degrees C is very limited. The need to measure sound speed in liquids up to 250 degrees C is of both fundamental interest, as in the case of basic equations of state, and applied interest, such as for characterizing geothermal or petroleum downhole environments. The measurement cell reported here represents an advancement in the established room temperature swept frequency acoustic interferometry measurement for liquid sound speed determinations. The paper details the selection of materials suitable for high temperature operation and the construction of the measurement apparatus. Representative sound speeds as a function of temperature and pressure are presented and are shown to be in very good agreement with an internationally accepted standard for water sound speed. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4765746] C1 [Sturtevant, Blake T.; Pantea, Cristian; Sinha, Dipen N.] Los Alamos Natl Lab, Los Alamos, NM 87544 USA. RP Sturtevant, BT (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87544 USA. EM bsturtev@lanl.gov RI Pantea, Cristian/D-4108-2009 FU (U.S.) Department of Energy (DOE) [AID 18832] FX This work was supported by the (U.S.) Department of Energy (DOE) under Award No. AID 18832. NR 22 TC 4 Z9 4 U1 3 U2 8 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0034-6748 J9 REV SCI INSTRUM JI Rev. Sci. Instrum. PD NOV PY 2012 VL 83 IS 11 AR 115106 DI 10.1063/1.4765746 PG 6 WC Instruments & Instrumentation; Physics, Applied SC Instruments & Instrumentation; Physics GA 050DY UT WOS:000312034400054 PM 23206097 ER PT J AU Vondrasek, R Delahaye, P Kutsaev, S Maunoury, L AF Vondrasek, R. Delahaye, P. Kutsaev, Sergey Maunoury, L. TI Improved charge breeding efficiency of light ions with an electron cyclotron resonance ion source SO REVIEW OF SCIENTIFIC INSTRUMENTS LA English DT Article AB The Californium Rare Isotope Breeder Upgrade is a new radioactive beam facility for the Argonne Tandem Linac Accelerator System (ATLAS). The facility utilizes a Cf-252 fission source coupled with an electron cyclotron resonance ion source to provide radioactive beam species for the ATLAS experimental program. The californium fission fragment distribution provides nuclei in the mid-mass range which are difficult to extract from production targets using the isotope separation on line technique and are not well populated by low-energy fission of uranium. To date the charge breeding program has focused on optimizing these mid-mass beams, achieving high charge breeding efficiencies of both gaseous and solid species including 14.7% for the radioactive species Ba-143(27+). In an effort to better understand the charge breeding mechanism, we have recently focused on the low-mass species sodium and potassium which up to present have been difficult to charge breed efficiently. Unprecedented charge breeding efficiencies of 10.1% for Na-23(7+) and 17.9% for K-39(10+) were obtained injecting stable Na+ and K+ beams from a surface ionization source. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4768533] C1 [Vondrasek, R.; Kutsaev, Sergey] Argonne Natl Lab, Argonne, IL 60439 USA. [Delahaye, P.; Maunoury, L.] CEA DSM CNRS IN2P3, GANIL, F-14076 Caen, France. RP Vondrasek, R (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. OI Kutsaev, Sergey/0000-0003-4996-2545 FU U.S. Department of Energy, Office of Nuclear Physics [DE-AC02-06CH11357]; European Union [262010] FX This work was supported by the U.S. Department of Energy, Office of Nuclear Physics, under Contract No. DE-AC02-06CH11357. The SPIRAL upgrade activities are supported by the European Union's Seventh Framework Programme under Grant Agreement No. 262010 within the ENSAR project, and within ERA-NET NuPNET as part of the EMILIE project. NR 16 TC 6 Z9 6 U1 2 U2 6 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0034-6748 J9 REV SCI INSTRUM JI Rev. Sci. Instrum. PD NOV PY 2012 VL 83 IS 11 AR 113303 DI 10.1063/1.4768533 PG 5 WC Instruments & Instrumentation; Physics, Applied SC Instruments & Instrumentation; Physics GA 050DY UT WOS:000312034400011 PM 23206054 ER PT J AU Weber, TE Slough, JT Kirtley, D AF Weber, T. E. Slough, J. T. Kirtley, D. TI The electrodeless Lorentz force (ELF) thruster experimental facility SO REVIEW OF SCIENTIFIC INSTRUMENTS LA English DT Article ID FIELD-REVERSED CONFIGURATIONS; CURRENT DRIVE; PLASMA; PENDULUM; STAND AB An innovative facility for testing high-power, pulsed plasmoid thrusters has been constructed to develop the electrodeless Lorentz force (ELF) thruster concept. It is equipped with a suite of diagnostics optimized to study the physical processes taking place within ELF and evaluate its propulsive utility including magnetic field, neutral gas, and plasma flux diagnostics, a method to determine energy flow into the plasma from the pulsed power systems, and a new type of ballistic pendulum, which enables thrust to be measured without the need for installing the entire propulsion system on a thrust stand. Variable magnetic fields allow controlled studies of plume expansion in a small-scale experiment and dielectric chamber walls reduce electromagnetic influences on plasma behavior and thruster operation. The unique capabilities of this facility enable novel concept development to take place at greatly reduced cost and increased accessibility compared to testing at large user-facilities. (C) 2012 American Institute of Physics. [http://dx.doi. org/10.1063/1.4759000] C1 [Weber, T. E.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Slough, J. T.; Kirtley, D.] MSNW LLC, Redmond, WA 98052 USA. RP Weber, TE (reprint author), Los Alamos Natl Lab, Mail Stop E526,POB 1663, Los Alamos, NM 87545 USA. FU STTR grant; Air Force Office of Scientific Research FX The authors wish to recognize the technical expertise of S. Andreason, C. Pihl, and G. Votroubek for their many contributions. T. Weber thanks T. Intrator for proofreading this manuscript. This work was funded by an STTR grant sponsored by the Air Force Office of Scientific Research. NR 33 TC 2 Z9 2 U1 1 U2 23 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0034-6748 J9 REV SCI INSTRUM JI Rev. Sci. Instrum. PD NOV PY 2012 VL 83 IS 11 AR 113509 DI 10.1063/1.4759000 PG 9 WC Instruments & Instrumentation; Physics, Applied SC Instruments & Instrumentation; Physics GA 050DY UT WOS:000312034400021 PM 23206064 ER PT J AU Chief, K Young, MH Shafer, DS AF Chief, Karletta Young, Michael H. Shafer, David S. TI Changes in Soil Structure and Hydraulic Properties in a Wooded-Shrubland Ecosystem following a Prescribed Fire SO SOIL SCIENCE SOCIETY OF AMERICA JOURNAL LA English DT Article ID WESTERN UNITED-STATES; PINYON-JUNIPER WOODLAND; WATER REPELLENCY; AIR PERMEABILITY; HYDROPHOBIC SUBSTANCES; TENSION INFILTROMETER; SEMIARID RANGELANDS; SPATIAL VARIABILITY; SEDIMENT PRODUCTION; ORGANIC-MATTER AB Pre- and post-fire measurements were made for a low-intensity prescribed fire in a semiarid, shrub-woodland transition zone, and objectives were to: (i) determine changes in near-saturated hydraulic conductivity (K-f measured with a tension infiltrometer), air permeability (k(a) measured with an air permeameter), and soil physical properties at shrub undercanopy and interspace microsites immediately before and after a fall burn and for a 13-mo period; and (ii) quantify the importance and effect of post-fire soil structure on hydraulic properties using pre- and post-fire measurements. At undercanopy microsites, structure deteriorated from a moderate to a weak subangular blocky structure after the fire that broke down to a structureless soil 10 mo later. At interspace microsites, post-fire soil structure deteriorated from a moderate-strong subangular blocky structure with hard dry consistency to a weak subangular blocky structure with soft dry consistency. After 10 mo, the intercanopy maintained a weak-moderate soil structure that became structureless-weak after 13 mo. Immediately after the fire, at both microsites, there was incomplete organic combustion, a decrease in bulk density, and an increase in k(a); however, at undercanopy microsites, there was no significant change in K-f even though there was a slight to moderate hydrophobicity, whereas at interspace microsites where no water repellency existed, K-f increased. These changes may be a result of expansion of vaporized water through soil pores that broke up aggregates, deteriorating soil structure. Thus, mechanisms that contributed to changes immediately and after the first year post-fire were different for low-intensity burns than for higher intensity burns. C1 [Chief, Karletta] Univ Arizona, Dep Soil Water & Environm Sci, Tucson, AZ 85721 USA. [Young, Michael H.] Univ Texas Austin, Bur Econ Geol, Jackson Sch Geosci, Austin, TX 78713 USA. [Shafer, David S.] DOE Off Legacy Management, Grand Junction, CO 81503 USA. RP Chief, K (reprint author), Univ Arizona, Dep Soil Water & Environm Sci, 1177 E 4th St,Shantz Bldg,Rm 429, Tucson, AZ 85721 USA. EM kchief@email.arizona.edu RI Young, Michael/J-8009-2012 OI Young, Michael/0000-0001-8479-9910 FU National Science Foundation Grants for Rapid Response Research [EAR-0952272]; U.S. Department of Energy National Nuclear Security Administration [DE-AC52-06NA26383]; DRI Research Advisory Council FX This research and publication was made possible through funding from the National Science Foundation Grants for Rapid Response Research (no. EAR-0952272), the U.S. Department of Energy National Nuclear Security Administration (Contract no. DE-AC52-06NA26383), and the DRI Research Advisory Council. We would also like to acknowledge John Healey and William Meyer for assisting in the field with tension infiltrometer measurements and Dr. Dave Dubois and Dr. George Nikolich for fire temperature measurements. In addition, the U.S. Bureau of Land Management (BLM), Ely (Nevada) District Office, provided permits for the field measurements and data on pre-fire fuel loads and vegetation composition. NR 122 TC 4 Z9 4 U1 0 U2 39 PU SOIL SCI SOC AMER PI MADISON PA 677 SOUTH SEGOE ROAD, MADISON, WI 53711 USA SN 0361-5995 J9 SOIL SCI SOC AM J JI Soil Sci. Soc. Am. J. PD NOV-DEC PY 2012 VL 76 IS 6 BP 1965 EP 1977 DI 10.2136/sssaj2012.0072 PG 13 WC Soil Science SC Agriculture GA 052EI UT WOS:000312180100005 ER PT J AU DeHoff, KJ Oostrom, M Zhang, C Grate, JW AF DeHoff, K. J. Oostrom, M. Zhang, C. Grate, J. W. TI Evaluation of Two-Phase Relative Permeability and Capillary Pressure Relations for Unstable Displacements in a Pore Network SO VADOSE ZONE JOURNAL LA English DT Article ID NONAQUEOUS-PHASE LIQUID; HETEROGENEOUS POROUS-MEDIA; CARBON-TETRACHLORIDE; FLOW BEHAVIOR; SCALE; SATURATION; MECHANISMS; MICROMODEL; FLUID; WATER AB At the pore scale, unstable displacement is often observed for two-fluid systems, depending on the capillary number and fluid viscosity ratio. At the continuum scale, unstable displacement is usually not considered. In this work, relations between nonwetting fluid relative permeabilities (k(rn)), fluid saturations (S-n), and capillary pressure heads (h(c)) are evaluated to predict average S-n values using a continuum-based simulator for displacements in a micromodel. To this end, a series of displacement experiments was conducted using five wetting nonwetting immiscible fluid pairs in a homogenous pore network. The micromodel was initially saturated with either polyethylene glycol 200 (PEG) or water as a wetting fluid, which was subsequently displaced by a nonwetting fluid (dodecane, hexadecane, or mineral oil) at different flow rates. Nonwetting fluid saturations increased with increasing flow rates for all five fluid pairs. Viscous fingering occurred when PEG was displaced by either dodecane or hexadecane. For the displacements of water, capillary fingers were observed at low capillary numbers. Fitting the experimental S-n and h(c), data with the BrooksCorey relationship indicated that the fitted and computed entry pressure heads, based on pore geometry and fluid properties, compare reasonably well. However, the fitted pore geometry factor values for these displacements are considerably lower than what is expected for displacements in homogeneous, highly uniform, porous systems, demonstrating the impact of unstable displacement. It was shown that a continuum-based multiphase simulator could be used to reasonably estimate the average S-n behavior for unstable wetting fluid displacement in a pore network as long as independently fitted h(c)-S-n and k(rn)-S-n relations were used. C1 [DeHoff, K. J.; Oostrom, M.] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99354 USA. [Zhang, C.; Grate, J. W.] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99354 USA. RP Oostrom, M (reprint author), Pacific NW Natl Lab, Energy & Environm Directorate, POB 999,MS K9-33, Richland, WA 99354 USA. EM mart.oostrom@pnnl.gov RI Zhang, Changyong/A-8012-2013 FU Pacific Northwest National Laboratory (PNNL) Directed Research and Development Program under PNNL's Carbon Sequestration Initiative; Battelle Memorial Institute for the Department of Energy (DOE) [DE-AC06-76RLO 1830]; DOE's Office of Biological and Environmental Research FX This research is supported by the Pacific Northwest National Laboratory (PNNL) Directed Research and Development Program under PNNL's Carbon Sequestration Initiative. PNNL is operated by the Battelle Memorial Institute for the Department of Energy (DOE) under Contract DE-AC06-76RLO 1830. The pore-scale experiments were performed in the Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by the DOE's Office of Biological and Environmental Research and located at PNNL. Scientists interested in conducting experimental work in the EMSL are encouraged to contact M. Oostrom (mart.oostrom@pnnl.gov). NR 47 TC 4 Z9 4 U1 0 U2 27 PU SOIL SCI SOC AMER PI MADISON PA 677 SOUTH SEGOE ROAD, MADISON, WI 53711 USA SN 1539-1663 J9 VADOSE ZONE J JI Vadose Zone J. PD NOV PY 2012 VL 11 IS 4 DI 10.2136/vzj2012.0024 PG 12 WC Environmental Sciences; Soil Science; Water Resources SC Environmental Sciences & Ecology; Agriculture; Water Resources GA 050VI UT WOS:000312082000037 ER PT J AU Haarder, EB Binley, A Looms, MC Doetsch, J Nielsen, L Jensen, KH AF Haarder, Eline B. Binley, Andrew Looms, Majken C. Doetsch, Joseph Nielsen, Lars Jensen, Karsten H. TI Comparing Plume Characteristics Inferred from Cross-Borehole Geophysical Data SO VADOSE ZONE JOURNAL LA English DT Article ID GROUND-PENETRATING RADAR; ELECTRICAL-RESISTIVITY TOMOGRAPHY; VADOSE ZONE; PREFERENTIAL FLOW; UNSATURATED FLOW; WATER-CONTENT; TRANSPORT; SANDSTONE; SOILS AB We compare results of three cross-borehole geophysical approaches for imaging tracer migration arising from a point injection of water in the unsaturated zone: three-dimensional electrical resistivity tomography (ERT), two-dimensional ground-penetrating radar (GPR) tomography and quasi-three-dimensional GPR tomography. In the studied field experiment, a tracer was injected for a period of 5 d and was monitored both during injection and for 5 d during the subsequent redistribution. The three methods show similar characteristics of the plume development and movement, which has a strong lateral component and slow vertical migration. In addition to revealing the main tracer plume, two-dimensional GPR and the quasi-three-dimensional GPR results show development of secondary plumes at depth, which are not captured by the three-dimensional ERT due to lack of resolution. The flow patterns are compared to geological information from a coring obtained at the site and it is concluded that the diversion of water in the lateral direction can be caused by a few thin layers of contrasting geological composition. Mass balance calculations based on moment analysis of the moisture content changes reveal that two-dimensional and quasi-three-dimensional GPR results show similar results and that three-dimensional ERT underestimate the amount of tracer substantially. Our results further show that the analysis volume as well as threshold value for moisture content increase has significant impact on computed mass recovery. The choice of threshold value, in particular, should be method-dependent and needs to be considered carefully if the results of the moment calculations are to be used in constraining hydrological models. C1 [Haarder, Eline B.; Looms, Majken C.; Nielsen, Lars; Jensen, Karsten H.] Univ Copenhagen, Dep Geog & Geol, DK-1168 Copenhagen, Denmark. [Doetsch, Joseph] Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA USA. [Binley, Andrew] Univ Lancaster, Lancaster Environm Ctr, Lancaster LA1 4YW, England. RP Haarder, EB (reprint author), Univ Copenhagen, Dep Geog & Geol, DK-1168 Copenhagen, Denmark. EM eh@geo.ku.dk RI Binley, Andrew/C-2487-2013; Looms, Majken/N-7471-2014; Jensen, Karsten/E-3469-2015; Nielsen, Lars/C-7142-2015; Doetsch, Joseph/A-9438-2008; OI Binley, Andrew/0000-0002-0938-9070; Looms, Majken/0000-0002-3831-6305; Jensen, Karsten/0000-0003-4020-0050; Nielsen, Lars/0000-0003-2024-2288; Doetsch, Joseph/0000-0002-2927-9557; Haarder, Eline/0000-0003-1396-3634 FU Hobe - Center for Hydrology FX Eline B. Haarder is funded by Hobe - Center for Hydrology (www.hobe.dk). The authors would also like to thank Rita Deiana and an anonymous reviewer for helpful contributions to the final manuscript. NR 37 TC 2 Z9 2 U1 0 U2 18 PU SOIL SCI SOC AMER PI MADISON PA 677 SOUTH SEGOE ROAD, MADISON, WI 53711 USA SN 1539-1663 J9 VADOSE ZONE J JI Vadose Zone J. PD NOV PY 2012 VL 11 IS 4 DI 10.2136/vzj2012.0031 PG 14 WC Environmental Sciences; Soil Science; Water Resources SC Environmental Sciences & Ecology; Agriculture; Water Resources GA 050VI UT WOS:000312082000038 ER PT J AU Jadoon, KZ Weihermuller, L Scharnagl, B Kowalsky, MB Bechtold, M Hubbard, SS Vereecken, H Lambot, S AF Jadoon, Khan Zaib Weihermueller, Lutz Scharnagl, Benedikt Kowalsky, Michael B. Bechtold, Michel Hubbard, Susan S. Vereecken, Harry Lambot, Sebastien TI Estimation of Soil Hydraulic Parameters in the Field by Integrated Hydrogeophysical Inversion of Time-Lapse Ground-Penetrating Radar Data SO VADOSE ZONE JOURNAL LA English DT Article ID WAVE-FORM INVERSION; BULK ELECTRICAL-CONDUCTIVITY; VOLUMETRIC WATER-CONTENT; RAINFALL-RUNOFF MODELS; DOMAIN REFLECTOMETRY; BOREHOLE RADAR; GEOPHYSICAL-DATA; GLOBAL OPTIMIZATION; UNSATURATED SOILS; IMMISCIBLE FLUIDS AB An integrated hydrogeophysical inversion approach was used to remotely infer the unsaturated soil hydraulic parameters from time-lapse ground-penetrating radar (GPR) data collected at a fixed location over a bare agricultural field. The GPR model combines a full-waveform solution of Maxwell's equations for three-dimensional wave propagation in planar layered media together with global reflection and transmission functions to account for the antenna and its interactions with the medium. The hydrological simulator HYDRUS-1D was used with a two layer single- and dual-porosity model. The radar model was coupled to the hydrodynamic model, such that the soil electrical properties (permittivity and conductivity) that serve as input to the GPR model become a function of the hydrodynamic model output (water content), thereby permitting estimation of the soil hydraulic parameters from the GPR data in an inversion loop. To monitor the soil water content dynamics, time-lapse GPR and time domain reflectometry (TDR) measurements were performed, whereby only GPR data was used in the inversion. Significant effects of water dynamics were observed in the time-lapse GPR data and in particular precipitation and evaporation events were clearly visible. The dual porosity model provided better results compared to the single porosity model for describing the soil water dynamics, which is supported by field observations of macropores. Furthermore, the GPR-derived water content profiles reconstructed from the integrated hydrogeophysical inversion were in good agreement with TDR observations. These results suggest that the proposed method is promising for non-invasive characterization of the shallow subsurface hydraulic properties and monitoring water dynamics at the field scale. C1 [Jadoon, Khan Zaib; Weihermueller, Lutz; Scharnagl, Benedikt; Bechtold, Michel; Vereecken, Harry; Lambot, Sebastien] Forschungszentrum Julich, Inst Bio & Geosci, Agrosphere IBG 3, D-52425 Julich, Germany. [Jadoon, Khan Zaib] KAUST, Water Desalinat & Reuse Ctr, Thuwal 239556900, Saudi Arabia. [Kowalsky, Michael B.; Hubbard, Susan S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Lambot, Sebastien] Catholic Univ Louvain, Earth & Life Inst, B-1348 Louvain, Belgium. RP Jadoon, KZ (reprint author), Forschungszentrum Julich, Inst Bio & Geosci, Agrosphere IBG 3, D-52425 Julich, Germany. EM k.z.jadoon@fz-juelich.de RI Jadoon, Khan/A-7524-2013; Hubbard, Susan/E-9508-2010; Bechtold, Michel/F-1870-2010 OI Bechtold, Michel/0000-0002-8042-9792 FU Forschungszentrum Julich GmbH (Germany); Universite catholique de Louvain; Fonds National de la Recherche Scientifique (UCL and FNRS, Belgium); Bundesministerium fur Bildung und Forschung (BMBF Germany); DOE [DE-AC0205CH11231] FX This work was supported by the Forschungszentrum Julich GmbH (Germany), the Universite catholique de Louvain and Fonds National de la Recherche Scientifique (UCL and FNRS, Belgium). Khan Zaib Jadoon was funded by the CROPSENSe project funded by Bundesministerium fur Bildung und Forschung (BMBF Germany). Support for Susan Hubbard and Michael Kowalsky was provided by DOE Contract DE-AC0205CH11231 to LBNL. The authors are grateful to Marc Grasmueck, two anonymous reviewers, and the associate editor for their efforts in improving the manuscript. NR 99 TC 22 Z9 22 U1 3 U2 52 PU SOIL SCI SOC AMER PI MADISON PA 677 SOUTH SEGOE ROAD, MADISON, WI 53711 USA SN 1539-1663 J9 VADOSE ZONE J JI Vadose Zone J. PD NOV PY 2012 VL 11 IS 4 DI 10.2136/vzj2011.0177 PG 17 WC Environmental Sciences; Soil Science; Water Resources SC Environmental Sciences & Ecology; Agriculture; Water Resources GA 050VI UT WOS:000312082000023 ER PT J AU Lu, ZM Kwicklis, EM AF Lu, Zhiming Kwicklis, Edward M. TI Numerical Evaluation of Effective Unsaturated Hydraulic Properties of Fractured Rocks using a Stochastic Continuum Approach SO VADOSE ZONE JOURNAL LA English DT Article ID EFFECTIVE FLOW BEHAVIOR; HETEROGENEOUS SOILS; POROUS-MEDIA; TRANSPORT; MODEL; CONDUCTIVITY; SANDS AB This study builds on past studies that have investigated the effective properties of unsaturated porous media and merges stochastic continuum concepts to develop a numerical procedure for estimating the effective flow parameters that are independent of pressure head or saturation. The procedure involves the development of a numerical permeameter based on randomly generated, spatially correlated fields of fundamental fracture properties such as spacing and aperture. Local values of hydraulic conductivity, and the van Genuchten fitting parameters alpha and n in this random field are computed from local values of mechanical aperture and spacing based on the cubic law and relationships established from pore-scale fracture simulations. By considering multiple realizations of these spatially correlated fields and by running the numerical permeameter over a range of effective saturations and flow rates, outputs are generated that can be fit with the standard van Genuchten model to estimate block effective values of saturated hydraulic conductivity and the van Genuchten unsaturated hydraulic parameters of a fracture continuum at the field scale. These parameters can then be incorporated to conventional numerical simulators originally developed for porous media. The study shows that reasonable approximations to the results obtained through computationally demanding stochastic simulations can be developed based on estimates of the mean fracture spacing and aperture. Although the example application assumes the presence of an impermeable rock matrix, the hydraulic properties estimated for the fracture continuum with this methodology can be combined with those measured or similarly estimated for a matrix continuum in dual-permeability continuum models. C1 [Lu, Zhiming; Kwicklis, Edward M.] Los Alamos Natl Lab, Computat Earth Sci Grp EES 16, Los Alamos, NM 87545 USA. RP Lu, ZM (reprint author), Los Alamos Natl Lab, Computat Earth Sci Grp EES 16, MS T003, Los Alamos, NM 87545 USA. EM zhiming@lanl.gov OI Lu, Zhiming/0000-0001-5800-3368 FU Department of Energy (DOE) FX This work was supported by Department of Energy (DOE) through Underground Test Area Projects. NR 22 TC 0 Z9 0 U1 0 U2 19 PU SOIL SCI SOC AMER PI MADISON PA 677 SOUTH SEGOE ROAD, MADISON, WI 53711 USA SN 1539-1663 J9 VADOSE ZONE J JI Vadose Zone J. PD NOV PY 2012 VL 11 IS 4 DI 10.2136/vzj2011.0164 PG 10 WC Environmental Sciences; Soil Science; Water Resources SC Environmental Sciences & Ecology; Agriculture; Water Resources GA 050VI UT WOS:000312082000016 ER PT J AU Mattigod, SV Bovaird, CC Wellman, DM Parker, KE Wood, MI AF Mattigod, Shas V. Bovaird, Chase C. Wellman, Dawn M. Parker, Kent E. Wood, Marc I. TI An Experimental Study of Diffusivity of Technetium-99 in Hanford Vadose Zone Sediments SO VADOSE ZONE JOURNAL LA English DT Article ID IRON AB One of the methods being considered at the Hanford site in the state of Washington for safely disposing of low-level radioactive wastes (LLW) is to encase the waste in concrete and entomb the packages in the Hanford vadose zone sediments. The current plan for waste isolation consists of stacking low-level waste packages on a trench floor, surrounding the stacks with reinforced steel, and encasing these packages with concrete. Any failure of the concrete encasement may result in water intrusion and consequent mobilization of radionuclides from the waste packages. The mobilized radionuclides may escape from the encased concrete by mass flow or diffusion and move into the surrounding subsurface sediments. It is therefore necessary to conduct an assessment of the performance of the concrete encasement structure and the surrounding soil's ability to retard radionuclide migration. Because of their anionic nature in aqueous solutions, the radionuclides, Tc-99 and I-129 were identified as long-term dose contributors in LLW. The leachability or diffusion of these radionuclide species must be measured to assess the long-term performance of waste grouts when contacted with vadose zone pore water or groundwater. To supplement the previously obtained data, a set of experiments were conducted using Tc-99-spiked concrete (with 0 or 4% metallic Fe additions) in contact with Hanford soil at extremely low moisture content (similar to 1% by mass). The Tc-99 diffusion profiles in the soil half-cells were measured a after a time lapse of similar to 1.9 yr and the diffusion coefficient was calculated to be similar to 1.0 x 10(-9) cm(2) s(-1). C1 [Mattigod, Shas V.; Bovaird, Chase C.; Wellman, Dawn M.; Parker, Kent E.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Wood, Marc I.] CH2M Hill Plateau Remediat Co, Richland, WA USA. RP Wellman, DM (reprint author), Pacific NW Natl Lab, POB 999, Richland, WA 99352 USA. EM Dawn.Wellman@pnnl.gov FU U.S. Department of Energy [DE-AC06-76RLO 1830]; CH2M Hill Plateau Remediation Company FX This study was supported by the U.S. Department of Energy under Contract DE-AC06-76RLO 1830. We thank Dr. Elizabeth Golovich of PNNL and Dr. Susan Hubbard, Co-Editor, for providing valuable comments. This study was supported by the CH2M Hill Plateau Remediation Company. NR 18 TC 0 Z9 0 U1 1 U2 21 PU SOIL SCI SOC AMER PI MADISON PA 677 SOUTH SEGOE ROAD, MADISON, WI 53711 USA SN 1539-1663 J9 VADOSE ZONE J JI Vadose Zone J. PD NOV PY 2012 VL 11 IS 4 DI 10.2136/vzj2011.0184 PG 5 WC Environmental Sciences; Soil Science; Water Resources SC Environmental Sciences & Ecology; Agriculture; Water Resources GA 050VI UT WOS:000312082000026 ER PT J AU Shi, XQ Ye, M Finsterle, S Wu, JC AF Shi, Xiaoqing Ye, Ming Finsterle, Stefan Wu, Jichun TI Comparing Nonlinear Regression and Markov Chain Monte Carlo Methods for Assessment of Prediction Uncertainty in Vadose Zone Modeling SO VADOSE ZONE JOURNAL LA English DT Article ID DIFFERENTIAL EVOLUTION; HYDRAULIC CONDUCTIVITY; 2-PHASE FLOW; SIMULATION; PARAMETERS; TRANSPORT; INTERVALS; INVERSE; CONFIDENCE; OPTIMIZATION AB In vadose zone modeling, parameter estimates and model predictions are inherently uncertain, regardless of quality and quantity of data used in model-data fusion. Accurate quantification of the uncertainty is necessary to design future data collection for improving the predictive capability of models. This study is focused on evaluating predictive performance of two commonly used methods of uncertainty quantification: nonlinear regression and Bayesian methods. The former quantifies predictive uncertainty using the regression confidence interval (RCI), whereas the latter uses the Bayesian credible interval (BCI); neither RCI nor BCI includes measurement errors. When measurement errors are considered, the counterparts of RCI and BCI are regression prediction interval (RPI) and Bayesian prediction interval (BPI), respectively. The predictive performance is examined through a cross-validation study of two-phase flow modeling, and predictive logscore is used as the performance measure. The linear and nonlinear RCI and RPI are evaluated using UCODE_2005. The nonlinear RCI performs better than the linear RCI, and the nonlinear RPI outperforms the linear RPI. The Bayesian intervals are calculated using Markov Chain Monte Carlo (MCMC) techniques implemented with the differential evolution adaptive metropolis (DREAM) algorithm. The BCI/BPI obtained from DREAM has better predictive performance than the linear and nonlinear RCI/RPI. Different from observations in other studies, it is found that estimating nonlinear RCI/RPI is not computationally more efficient than estimating BCl/BPI in this case with low-dimensional parameter space and a large number of predictions. MCMC methods are thus more appealing than nonlinear regression methods for uncertainty quantification in vadose zone modeling. C1 [Shi, Xiaoqing; Ye, Ming] Florida State Univ, Dep Sci Comp, Tallahassee, FL 32306 USA. [Shi, Xiaoqing; Ye, Ming] Florida State Univ, Geophys Fluid Dynam Inst, Tallahassee, FL 32306 USA. [Finsterle, Stefan] Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Shi, Xiaoqing; Wu, Jichun] Nanjing Univ, Dep Hydrosci, Nanjing 210098, Jiangsu, Peoples R China. RP Ye, M (reprint author), Florida State Univ, Dep Sci Comp, Tallahassee, FL 32306 USA. EM mye@fsu.edu RI Ye, Ming/A-5964-2008; Finsterle, Stefan/A-8360-2009; Shi, Xiaoqing/G-4439-2010 OI Finsterle, Stefan/0000-0002-4446-9906; Shi, Xiaoqing/0000-0002-5074-8856 FU NSF-EAR [0911074]; DOE-SBR [DE-SC0002687]; ORAU/ORNL; National Science Foundation of China [41172206, 40725010, 41030746]; U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported in part by NSF-EAR grant 0911074, DOE-SBR grant DE-SC0002687, and ORAU/ORNL High Performance Computing Grant. The first and last authors are also supported by the National Science Foundation of China (No. 41172206, 40725010 and 41030746). The third author was supported, in part, by the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The authors thank Jasper Vrugt for providing the DREAM code and Mary Hill for discussion on calculation of nonlinear confidence intervals. NR 73 TC 7 Z9 7 U1 7 U2 44 PU SOIL SCI SOC AMER PI MADISON PA 677 SOUTH SEGOE ROAD, MADISON, WI 53711 USA SN 1539-1663 J9 VADOSE ZONE J JI Vadose Zone J. PD NOV PY 2012 VL 11 IS 4 DI 10.2136/vzj2011.0147 PG 16 WC Environmental Sciences; Soil Science; Water Resources SC Environmental Sciences & Ecology; Agriculture; Water Resources GA 050VI UT WOS:000312082000011 ER PT J AU Stauffer, PH Lu, ZM AF Stauffer, Philip H. Lu, Zhiming TI Quantifying Transport Uncertainty in Unsaturated Rock using Monte Carlo Sampling of Retention Curves SO VADOSE ZONE JOURNAL LA English DT Article ID BREAKTHROUGH CURVES; YUCCA MOUNTAIN; POROUS-MEDIA; LOS-ALAMOS; NEW-MEXICO; SITE; MODELS; FLOW; AQUIFER; SCALE AB We have developed a new Monte Carlo sampling method for simulating flow and transport in unsaturated porous media, characterized by van Genuchten-Mualem constitutive relations. Instead of sampling each individual soil parameter from its probability space and then running Monte Carlo simulations using realizations of rock parameters directly, we calculate retention curves from realizations of rock parameters, take subsamples from these retention curves, and run simulations using parameter realizations corresponding to these selected retention curves. The retention curve subsampling methodology was applied to three-dimensional simulations of conservative tracer transport beneath Material Disposal Area G at the Los Alamos National Laboratory. Convergence of the proposed sampling method was assessed by comparing statistics of breakthrough curves observed at a compliance boundary with those obtained using between 25 and 1000 Latin hypercube sampling (LHS) Monte Carlo simulations. Our example shows that 25 model runs based on selected retention curves could adequately approximate the results from our assumed truth (1000 LHS Monte Carlo simulations), while LHS alone required in excess of 50 realizations to achieve the same quality result. Another finding from this work is that the median of the breakthrough curves was more meaningful than the arithmetic mean of curves, and the former was nearly identical to the breakthrough curve derived from mean rock properties. C1 [Stauffer, Philip H.; Lu, Zhiming] Los Alamos Natl Lab, Computat Earth Sci Grp EES 16, Los Alamos, NM 87545 USA. RP Stauffer, PH (reprint author), Los Alamos Natl Lab, Computat Earth Sci Grp EES 16, POB 1663, Los Alamos, NM 87545 USA. EM stauffer@lanl.gov OI Stauffer, Philip/0000-0002-6976-221X; Lu, Zhiming/0000-0001-5800-3368 FU Performance Assessment for MDA G, Los Alamos National Laboratory under from the U.S. Department of Energy FX This study was supported by the Performance Assessment for MDA G, Los Alamos National Laboratory, under funding from the U.S. Department of Energy. We thank Rob Shuman for helpful review of the material. We also gratefully acknowledge the thoughtful reviews of two anonymous reviewers. NR 33 TC 2 Z9 2 U1 1 U2 4 PU SOIL SCI SOC AMER PI MADISON PA 677 SOUTH SEGOE ROAD, MADISON, WI 53711 USA SN 1539-1663 J9 VADOSE ZONE J JI Vadose Zone J. PD NOV PY 2012 VL 11 IS 4 DI 10.2136/vzj2011.0171 PG 13 WC Environmental Sciences; Soil Science; Water Resources SC Environmental Sciences & Ecology; Agriculture; Water Resources GA 050VI UT WOS:000312082000020 ER PT J AU Szecsody, JE Truex, MJ Zhong, L Johnson, TC Qafoku, NP Williams, MD Greenwood, WJ Wallin, EL Bargar, JD Faurie, DK AF Szecsody, J. E. Truex, M. J. Zhong, L. Johnson, T. C. Qafoku, N. P. Williams, M. D. Greenwood, W. J. Wallin, E. L. Bargar, J. D. Faurie, D. K. TI Geochemical and Geophysical Changes during Ammonia Gas Treatment of Vadose Zone Sediments for Uranium Remediation SO VADOSE ZONE JOURNAL LA English DT Article ID CONTAMINATED SEDIMENTS; URANYL-CARBONATE; HANFORD-SITE; DISSOLUTION; PRECIPITATION; EXTRACTION; MINERALS; CANCRINITE; RETENTION; TRANSPORT AB Low water content sediments were treated with NH3 gas to evaluate changes in U mobility as a potential field remediation method for vadose zone contamination. Injection of NH3 gas created high dissolved NH3 concentrations that followed equilibrium behavior. High NH3 concentration led to an increase in pH from 8.0 to 11 to 13, depending on the water content and NH3 concentration. The increase in pore water pH resulted in a large increase in pore water cations and anions from mineral-phase dissolution. Minerals showing the greatest dissolution included montmorillonite, muscovite, and kaolinite. Pore water ion concentrations then decreased with time. Simulations based on initial pore water ion concentrations indicated that quartz, chrysotile, calcite, diaspore, hematite, and Na-boltwoodite (hydrous U silicate) should precipitate. Electrical resistivity and induced polarization tomography (ERT/IP) was able to nonintrusively track these NH3 partitioning, dissolution, and precipitations processes through changes in conductivity and chargeability. Ammonia treatment significantly decreases the amount of U present as adsorbed and aqueous species in field-contaminated sediments. In contrast, sediments containing a large fraction of U associated with carbonates generally showed little change. Uranium leaching from sediments containing high Na-boltwoodite decreased significantly by NH3 treatment, but x-ray absorption near-edge structure/extended x-ray absorption fine structure showed no change in the Na-boltwoodite concentration. Therefore, NH3 treatment of contaminated sediment acts to decrease the highly mobile aqueous and adsorbed U by incorporation into precipitates and appears to decrease mobility of some existing U precipitates (Na-boltwoodite) as a result of mineral coating. C1 [Szecsody, J. E.; Truex, M. J.; Zhong, L.; Johnson, T. C.; Qafoku, N. P.; Williams, M. D.; Greenwood, W. J.; Wallin, E. L.; Bargar, J. D.; Faurie, D. K.] Pacific NW Natl Lab, Richland, WA 99354 USA. RP Szecsody, JE (reprint author), Pacific NW Natl Lab, POB 999,MS K3-61, Richland, WA 99354 USA. EM jim.szecsody@pnnl.gov OI Qafoku, Nikolla P./0000-0002-3258-5379 FU CH2M Hill Plateau Remediation Company, Richland, WA; Department of Energy [DE-AC06-76RLO 1830] FX Funding for this research was provided by CH2M Hill Plateau Remediation Company, Richland, WA. Pacific Northwest National is operated by the Battelle Memorial Institute for the Department of Energy under Contract DE-AC06-76RLO 1830. NR 33 TC 4 Z9 4 U1 0 U2 18 PU SOIL SCI SOC AMER PI MADISON PA 677 SOUTH SEGOE ROAD, MADISON, WI 53711 USA SN 1539-1663 J9 VADOSE ZONE J JI Vadose Zone J. PD NOV PY 2012 VL 11 IS 4 DI 10.2136/vzj2011.0158 PG 13 WC Environmental Sciences; Soil Science; Water Resources SC Environmental Sciences & Ecology; Agriculture; Water Resources GA 050VI UT WOS:000312082000014 ER PT J AU Truex, MJ Oostrom, M Strickland, CE Chronister, GB Benecke, MW Johnson, CD AF Truex, M. J. Oostrom, M. Strickland, C. E. Chronister, G. B. Benecke, M. W. Johnson, C. D. TI Field-Scale Assessment of Desiccation Implementation for Deep Vadose Zone Contaminants SO VADOSE ZONE JOURNAL LA English DT Article ID SOIL-WATER RETENTION; UNSATURATED POROUS-MEDIA; HYDRAULIC CONDUCTIVITY; CALIBRATION AB Desiccation of the vadose zone has the potential to reduce the flux of contaminants to underlying groundwater by removing moisture and decreasing the water relative permeability of the desiccated zone. However, data to evaluate implementation of desiccation are needed before desiccation can be considered as a potential remedy. Implementation of desiccation was field tested by injecting dry nitrogen gas to a target treatment zone and monitoring the spatial and temporal progress of the drying process. Aqueous waste discharges to disposal cribs approximately 50 yr ago distributed water and contaminants, primarily technetium-99 and nitrate, within the 100-m deep vadose zone at the test site. The test was conducted adjacent to one of the former disposal cribs in a contaminated portion of the vadose zone dominated by fine sands with lenses of loamy sand. Desiccation removed over 18,000 kg of water from the test zone within the 151-d active desiccation period and reduced volumetric moisture content over 1300 m(3) of soil with values lower than 0.01 (m(3) m(-3)) in 68 m(3). The lateral and vertical distribution of drying from the injection well was influenced by the sub-surface heterogeneity with initial drying in higher permeability zones. However, over time, desiccation also occurred in the initially wetter, lower permeability lenses. C1 [Truex, M. J.; Oostrom, M.; Strickland, C. E.; Johnson, C. D.] Pacific NW Natl Lab, Div Energy & Environm, Richland, WA 99354 USA. [Chronister, G. B.; Benecke, M. W.] CH2M Hill Plateau Remediat Co, Richland, WA 99352 USA. RP Truex, MJ (reprint author), Pacific NW Natl Lab, Div Energy & Environm, POB 999,MS K6-96, Richland, WA 99354 USA. EM mj.truex@pnl.gov FU CH2M Hill Plateau Remediation Company, Richland, WA; Department of Energy (DOE) [DE-AC06-76RLO 1830] FX Funding for this research was provided by CH2M Hill Plateau Remediation Company, Richland, WA. Pacific Northwest National Laboratory is operated by the Battelle Memorial Institute for the Department of Energy (DOE) under Contract DE-AC06-76RLO 1830. Neutron logging was conducted by the S.M. Stoller Corporation, Hanford Office, under contract to CH2M Hill Plateau Remediation Company, Richland, WA. NR 26 TC 5 Z9 5 U1 3 U2 27 PU SOIL SCI SOC AMER PI MADISON PA 677 SOUTH SEGOE ROAD, MADISON, WI 53711 USA SN 1539-1663 J9 VADOSE ZONE J JI Vadose Zone J. PD NOV PY 2012 VL 11 IS 4 DI 10.2136/vzj2011.0144 PG 10 WC Environmental Sciences; Soil Science; Water Resources SC Environmental Sciences & Ecology; Agriculture; Water Resources GA 050VI UT WOS:000312082000008 ER PT J AU Wellman, DM Freshley, MD Johnson, TC Miracle, AL AF Wellman, Dawn M. Freshley, Mark D. Johnson, Tim C. Miracle, Ann L. TI Contaminants in Vadose Zone Environments SO VADOSE ZONE JOURNAL LA English DT Article AB Contaminants in vadose zone environments pose a long-term source and threat to groundwater resources, human health, and the environment. A number of technical, regulatory, and policy challenges and opportunities are associated with contamination in vadose zone environments, particularly in remediation. In this special section, 12 papers present novel approaches to characterize, monitor, remediate, and predict the transport and fate of contaminants in vadose zone environments. C1 [Wellman, Dawn M.; Freshley, Mark D.; Johnson, Tim C.; Miracle, Ann L.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Wellman, DM (reprint author), Pacific NW Natl Lab, 902 Battelle Blvd, Richland, WA 99352 USA. EM dawn.wellman@pnnl.gov NR 6 TC 0 Z9 0 U1 1 U2 9 PU SOIL SCI SOC AMER PI MADISON PA 677 SOUTH SEGOE ROAD, MADISON, WI 53711 USA SN 1539-1663 J9 VADOSE ZONE J JI Vadose Zone J. PD NOV PY 2012 VL 11 IS 4 DI 10.2136/vzj2012.0159 PG 3 WC Environmental Sciences; Soil Science; Water Resources SC Environmental Sciences & Ecology; Agriculture; Water Resources GA 050VI UT WOS:000312082000045 ER PT J AU Wu, YX Hubbard, S Wellman, D AF Wu, Yuxin Hubbard, Susan Wellman, Dawn TI Geophysical Monitoring of Foam Used to Deliver Remediation Treatments within the Vadose Zone SO VADOSE ZONE JOURNAL LA English DT Article ID INDUCED-POLARIZATION; ELECTRICAL-RESISTIVITY; AIR/WATER INTERFACE; SEDIMENTS; BIOREMEDIATION; PERFORMANCE; RADAR; MODEL; SANDS AB Foam is a promising vehicle for delivering amendments into the vadose zone for in situ remediation; it is an approach being considered for in situ treatment and stabilization of metals and radionuclides located within the deep vadose zone of the Department of Energy's Hanford Site in the state of Washington. A central aspect of evaluating the effectiveness of this approach is the ability to monitor foam distribution, its transformation, and the reactions that it induces in the subsurface, ideally in a noninvasive manner. In this study, we performed laboratory experiments to evaluate the potential of geophysical methods (complex resistivity and time-domain reflectometry [TDRI) as tools for monitoring foam-assisted amendment delivery in the deep vadose zone. Our results indicated great sensitivity of electrical methods to foam transportation and evolution in unsaturated porous media that were related to foam bubble coalescence and drainage processes. Specifically, we observed (i) a decrease in electrical resistivity (increase in electrical conductivity) by more than an order of magnitude in both silica sand and natural sediment matrices during foam transportation; (ii) an increase in resistivity (decrease in conductivity) of more than twofold during foam coalescence and drainage; and (iii) a distinct phase and imaginary conductivity signature related to the evolution of water films on sediment grains during foam injection and evolution processes. To assist with the interpretation of these data, TDR measurements were used to monitor moisture content, which provided complementary information about foam distribution and drainage. Our results clearly demonstrated the sensitivity of electrical and TDR signals to foam transportation and evolution in unsaturated porous media and suggest the potential of these methods for monitoring the response of a system to foam-based remediation treatments at field scales. C1 [Wu, Yuxin; Hubbard, Susan] Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Wellman, Dawn] Pacific NW Natl Lab, Environm Syst Grp, Richland, WA 99352 USA. RP Wu, YX (reprint author), Lawrence Berkeley Natl Lab, Div Earth Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM ywu3@lbl.gov RI Hubbard, Susan/E-9508-2010; Wu, Yuxin/G-1630-2012 OI Wu, Yuxin/0000-0002-6953-0179 FU U.S. Department of Energy, Office of Environmental Management; U.S. Department of Energy, EM-30 Technology Innovation and Development Office; Richland Operations Office FX This research was supported by the U.S. Department of Energy, Office of Environmental Management, EM-30 Technology Innovation and Development Office, and Richland Operations Office. Help from Elsa Cordova and Danielle Jansik at PNNL on site sediments and foam generation method is highly appreciated. We thank the associate editor Andrew Ramsburg. We also thank Dale Rucker and two anonymous reviewers for constructive comments. NR 42 TC 0 Z9 0 U1 3 U2 12 PU SOIL SCI SOC AMER PI MADISON PA 677 SOUTH SEGOE ROAD, MADISON, WI 53711 USA SN 1539-1663 J9 VADOSE ZONE J JI Vadose Zone J. PD NOV PY 2012 VL 11 IS 4 DI 10.2136/vzj2011.0160 PG 12 WC Environmental Sciences; Soil Science; Water Resources SC Environmental Sciences & Ecology; Agriculture; Water Resources GA 050VI UT WOS:000312082000015 ER PT J AU Zhang, ZF Zhong, LR White, MD Szecsody, JE AF Zhang, Z. Fred Zhong, Lirong White, Mark D. Szecsody, James E. TI Experimental Investigation of the Effective Foam Viscosity in Unsaturated Porous Media SO VADOSE ZONE JOURNAL LA English DT Article ID CONTAMINATED SOIL; SURFACTANT FOAM; VADOSE ZONE; REMEDIATION; PROPAGATION; TECHNOLOGY; DELIVERY AB Foam has the potential to effectively carry and distribute either aqueous or gaseous amendments to the deep vadose zone for contaminant remediation. However, the transport of foam in porous media is complicated because flow characteristics such as effective viscosity are affected not only by foam properties but also by the sediment properties and flow conditions. We determined the average effective foam viscosity via a series of laboratory experiments and found that the effective foam viscosity was significantly higher than the viscosity of gas or water and increased with the liquid fraction in foam, the injection rate, and sediment permeability. These impacts are successfully described with a mathematical expression, which is further demonstrated with data from the literature. These results suggest that, when foam is used in deep vadose zone remediation, foam flow is almost not affected by gravity and is capable of distributing amendments uniformly in heterogeneous sediments. C1 [Zhang, Z. Fred; Zhong, Lirong; White, Mark D.; Szecsody, James E.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Zhang, ZF (reprint author), Pacific NW Natl Lab, 902 Batelle Blvd, Richland, WA 99352 USA. EM fred.zhang@pnnl.gov FU U.S. Department of Energy Office of Environmental Management; Richland Operations Office; Battelle Memorial Institute for the Department of Energy (DOE) [DE-AC05-76RL01830] FX Funding for this work was provided by the U.S. Department of Energy Office of Environmental Management and Richland Operations Office. The Pacific Northwest National Laboratory is operated by Battelle Memorial Institute for the Department of Energy (DOE) under Contract DE-AC05-76RL01830. NR 16 TC 2 Z9 2 U1 2 U2 9 PU SOIL SCI SOC AMER PI MADISON PA 677 SOUTH SEGOE ROAD, MADISON, WI 53711 USA SN 1539-1663 J9 VADOSE ZONE J JI Vadose Zone J. PD NOV PY 2012 VL 11 IS 4 DI 10.2136/vzj2011.0190 PG 9 WC Environmental Sciences; Soil Science; Water Resources SC Environmental Sciences & Ecology; Agriculture; Water Resources GA 050VI UT WOS:000312082000028 ER PT J AU Zhong, LR Oostrom, M AF Zhong, Lirong Oostrom, Mart TI LNAPL Removal from Unsaturated Porous Media Using Surfactant Infiltration SO VADOSE ZONE JOURNAL LA English DT Article ID NONAQUEOUS PHASE LIQUIDS; REMEDIAL AMENDMENT DELIVERY; ENHANCED REMEDIATION; CONTAMINATED SOIL; SUBSURFACE; WATER; SOLUBILIZATION; ADSORPTION; CHEMISTRY; PRESSURE AB A series of unsaturated column experiments was conducted to evaluate light nonaqueous phase liquid (LNAPL) removal during surfactant solution infiltration. Surfactant-LNAPL phase behavior tests were conducted to optimize the remedial solutions. Packed sand and site sediment columns were first processed to establish representative LNAPL smear zones under unsaturated conditions. Infiltration of low-concentration surfactant was then applied in a stepwise flush mode, with 0.33 column pore volume (PV) of solution in each flush. The influence of infiltrated surfactant solution volume and pH on LNAPL removal was assessed. A LNAPL bank was observed at the front of the first surfactant infiltration in each column, indicating that a very low surfactant concentration is needed to reduce the LNAPL-water interfacial tension sufficiently to mobilize trapped LNAPL under unsaturated conditions. More LNAPL was recovered as additional steps of surfactant infiltration were applied. Up to 99% LNAPL was removed after six infiltration steps, with approximately 2.0 PV of total surfactant solution application, suggesting surfactant infiltration may be an effective method for vadose zone LNAPL remediation. The influence of pH tested in this study (3.99 similar to 10.85) was insignificant because the buffering capacity of the sediment kept the pH in the column higher than the zero point charge (pH(zp)) of the sediment and therefore surfactant sorption was negligible. C1 [Zhong, Lirong; Oostrom, Mart] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. RP Zhong, LR (reprint author), Pacific NW Natl Lab, Energy & Environm Directorate, 902 Battle Bvld,POB 999,MSIN K6-96, Richland, WA 99352 USA. EM lirong.zhong@pnnl.gov FU Pacific Northwest National Laboratory (PNNL); University of Texas at Austin; US Department of Energy [DE-AC06-76RLO 1830] FX This work is supported by grants from the Pacific Northwest National Laboratory (PNNL) and University of Texas at Austin. We thank Dr. Gary Pope at the University of Texas at Austin for his support in this research. PNNL is operated by Battelle for the US Department of Energy under contract DE-AC06-76RLO 1830. NR 39 TC 1 Z9 1 U1 3 U2 22 PU SOIL SCI SOC AMER PI MADISON PA 677 SOUTH SEGOE ROAD, MADISON, WI 53711 USA SN 1539-1663 J9 VADOSE ZONE J JI Vadose Zone J. PD NOV PY 2012 VL 11 IS 4 DI 10.2136/vzj2011.0166 PG 8 WC Environmental Sciences; Soil Science; Water Resources SC Environmental Sciences & Ecology; Agriculture; Water Resources GA 050VI UT WOS:000312082000017 ER PT J AU Cich, MJ McRaven, CP Lopez, GV Sears, TJ Hurtmans, D Mantz, AW AF Cich, M. J. McRaven, C. P. Lopez, G. V. Sears, T. J. Hurtmans, D. Mantz, A. W. TI Temperature-dependent pressure broadened line shape measurements in the nu (1)+nu (3) band of acetylene using a diode laser referenced to a frequency comb SO APPLIED PHYSICS B-LASERS AND OPTICS LA English DT Article ID MULTISPECTRUM ANALYSIS; COLLISIONAL WIDTH; TITANS ATMOSPHERE; SPECTRAL LINES; AR; DOPPLER; N-2; HE; SPECTROSCOPY; PARAMETERS AB Using an extended cavity diode laser referenced to a femtosecond frequency comb, the P(11) absorption line in the nu (1)+nu (3) combination band of the most abundant isotopologue of pure acetylene was studied at temperatures of 296, 240, 200, 175, 165, 160, 155, and 150 K to determine pressure-dependent line shape parameters at these temperatures. The laser emission profile, the instrumental resolution, is a Lorentz function characterized by a half width at half the maximum emission (HWHM) of 8.3x10(-6) cm(-1) (or 250 kHz) for these measurements. Six collision models were tested in fitting the experimental data: Voigt, speed-dependent Voigt, Rautian-Sobel'man, Galatry, and two Rautian-Galatry hybrid models (with and without speed-dependence). Only the speed-dependent Voigt model was able to fit the data to the experimental noise level at all temperatures and for pressures between 3 and nearly 360 torr. The variations of the speed-dependent Voigt profile line shape parameters with temperature were also characterized, and this model accurately reproduces the observations over their entire range of temperature and pressure. C1 [Cich, M. J.; Lopez, G. V.; Sears, T. J.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [McRaven, C. P.; Sears, T. J.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Hurtmans, D.] Univ Libre Brussels, Serv Chim Quant & Photophys Atomes Mol & Atmosphe, B-10050 Brussels, Belgium. [Mantz, A. W.] Connecticut Coll, Dept Phys Astron & Astrophys, New London, CT 06320 USA. RP Sears, TJ (reprint author), SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. EM trevor.sears@stonybrook.edu FU American Chemical Society; Brookhaven National Laboratory; DOE EPSCoR [DOE-07ER46361]; NASA EPSCoR [PS 4990]; NASA [NNX09AJ93G, NNX08AO78G]; US Department of Energy, Office of Science [DE-AC02-98CH10886]; Division of Chemical Sciences, Geosciences and Biosciences within the Office of Basic Energy Sciences FX Acknowledgment is made to the Donors of the American Chemical Society Petroleum Research Fund for partial support of this research. We are grateful for Program Development Funding awarded to TJS by Brookhaven National Laboratory which provided funds for some of the equipment used in this work. CPM gratefully acknowledges support by DOE EPSCoR grant DOE-07ER46361 for work conducted at the University of Oklahoma. AWM gratefully acknowledges support by NASA EPSCoR Grant No. PS 4990 for supporting the development of low temperature cells. The measurements and analyses were performed under grants NNX09AJ93G and NNX08AO78G from the NASA Planetary and Atmospheres program. Work at Brookhaven National Laboratory was carried out under Contract No. DE-AC02-98CH10886 with the US Department of Energy, Office of Science, and supported by its Division of Chemical Sciences, Geosciences and Biosciences within the Office of Basic Energy Sciences. NR 38 TC 10 Z9 10 U1 1 U2 20 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0946-2171 J9 APPL PHYS B-LASERS O JI Appl. Phys. B-Lasers Opt. PD NOV PY 2012 VL 109 IS 3 BP 373 EP 384 DI 10.1007/s00340-011-4829-0 PG 12 WC Optics; Physics, Applied SC Optics; Physics GA 050VF UT WOS:000312081700002 ER PT J AU Bachelet, E Fouque, P Han, C Gould, A Albrow, MD Beaulieu, JP Bertin, E Bond, IA Christie, GW Heyrovsky, D Horne, K Jorgensen, UG Maoz, D Mathiasen, M Matsunaga, N McCormick, J Menzies, J Nataf, D Natusch, T Oi, N Renon, N Tsapras, Y Udalski, A Yee, JC Batista, V Bennett, DP Brillant, S Caldwell, JAR Cassan, A Cole, A Cook, KH Coutures, C Dieters, S Dominik, M Prester, DD Donatowicz, J Greenhill, J Kains, N Kane, SR Marquette, JB Martin, R Pollard, KR Sahu, KC Street, RA Wambsganss, J Williams, A Zub, M Bos, M Dong, SB Drummond, J Gaudi, BS Graff, D Janczak, J Kaspi, S Kozlowski, S Lee, CU Monard, LAG Munoz, JA Park, BG Pogge, RW Polishook, D Shporer, A Abe, F Botzler, CS Fukui, A Furusawa, K Hearnshaw, JB Itow, Y Korpela, AV Ling, CH Masuda, K Matsubara, Y Miyake, N Muraki, Y Ohnishi, K Rattenbury, NJ Saito, T Sullivan, D Sumi, T Suzuki, D Sweatman, WL Tristram, PJ Wada, K Allan, A Bode, MF Bramich, DM Clay, N Fraser, SN Hawkins, E Kerins, E Lister, TA Mottram, CJ Saunders, ES Snodgrass, C Steele, IA Wheatley, PJ Bozza, V Browne, P Burgdorf, MJ Novati, SC Dreizler, S Finet, F Glitrup, M Grundahl, F Harpsoe, K Hessman, FV Hinse, TC Hundertmark, M Liebig, C Maier, G Mancini, L Rahvar, S Ricci, D Scarpetta, G Skottfelt, J Southworth, J Surdej, J Zimmer, F AF Bachelet, E. Fouque, P. Han, C. Gould, A. Albrow, M. D. Beaulieu, J. -P. Bertin, E. Bond, I. A. Christie, G. W. Heyrovsky, D. Horne, K. Jorgensen, U. G. Maoz, D. Mathiasen, M. Matsunaga, N. McCormick, J. Menzies, J. Nataf, D. Natusch, T. Oi, N. Renon, N. Tsapras, Y. Udalski, A. Yee, J. C. Batista, V. Bennett, D. P. Brillant, S. Caldwell, J. A. R. Cassan, A. Cole, A. Cook, K. H. Coutures, C. Dieters, S. Dominik, M. Prester, D. Dominis Donatowicz, J. Greenhill, J. Kains, N. Kane, S. R. Marquette, J. -B. Martin, R. Pollard, K. R. Sahu, K. C. Street, R. A. Wambsganss, J. Williams, A. Zub, M. Bos, M. Dong, Subo Drummond, J. Gaudi, B. S. Graff, D. Janczak, J. Kaspi, S. Kozlowski, S. Lee, C. -U. Monard, L. A. G. Munoz, J. A. Park, B. -G. Pogge, R. W. Polishook, D. Shporer, A. Abe, F. Botzler, C. S. Fukui, A. Furusawa, K. Hearnshaw, J. B. Itow, Y. Korpela, A. V. Ling, C. H. Masuda, K. Matsubara, Y. Miyake, N. Muraki, Y. Ohnishi, K. Rattenbury, N. J. Saito, To. Sullivan, D. Sumi, T. Suzuki, D. Sweatman, W. L. Tristram, P. J. Wada, K. Allan, A. Bode, M. F. Bramich, D. M. Clay, N. Fraser, S. N. Hawkins, E. Kerins, E. Lister, T. A. Mottram, C. J. Saunders, E. S. Snodgrass, C. Steele, I. A. Wheatley, P. J. Bozza, V. Browne, P. Burgdorf, M. J. Novati, S. Calchi Dreizler, S. Finet, F. Glitrup, M. Grundahl, F. Harpsoe, K. Hessman, F. V. Hinse, T. C. Hundertmark, M. Liebig, C. Maier, G. Mancini, L. Rahvar, S. Ricci, D. Scarpetta, G. Skottfelt, J. Southworth, J. Surdej, J. Zimmer, F. CA PLANET Collaboration FUN Collaboration MOA Collaboration RoboNet-II Collaboration MiNDSTEp Consortium TI A brown dwarf orbiting an M-dwarf: MOA 2009-BLG-411L SO ASTRONOMY & ASTROPHYSICS LA English DT Article DE binaries: general; gravitational lensing: micro; stars: individual: MOA 2009-BLG-411L ID MAGNIFICATION MICROLENSING EVENTS; SURFACE BRIGHTNESS RELATIONS; DIFFERENCE IMAGE-ANALYSIS; CLUMP ABSOLUTE MAGNITUDE; GALACTIC BULGE FIELDS; INTERSTELLAR EXTINCTION; BINARY INTERPRETATIONS; CENTRAL PERTURBATIONS; PLANETARY SYSTEMS; MASS PLANET AB Context. Caustic crossing is the clearest signature of binary lenses in microlensing. In the present context, this signature is diluted by the large source star but a detailed analysis has allowed the companion signal to be extracted. Aims. MOA 2009-BLG-411 was detected on August 5, 2009 by the MOA-Collaboration. Alerted as a high-magnification event, it was sensitive to planets. Suspected anomalies in the light curve were not confirmed by a real-time model, but further analysis revealed small deviations from a single lens extended source fit. Methods. Thanks to observations by all the collaborations, this event was well monitored. We first decided to characterize the source star properties by using a more refined method than the classical one: we measure the interstellar absorption along the line of sight in five different passbands (VIJHK). Secondly, we model the lightcurve by using the standard technique: make (s, q, alpha) grids to look for local minima and refine the results by using a downhill method (Markov chain Monte Carlo). Finally, we use a Galactic model to estimate the physical properties of the lens components. Results. We find that the source star is a giant G star with radius 9 R-circle dot. The grid search gives two local minima, which correspond to the theoretical degeneracy s = s(-1). We find that the lens is composed of a brown dwarf secondary of mass M-S = 0.05 M-circle dot orbiting a primary M-star of mass M-P = 0.18 M-circle dot. We also reveal a new mass-ratio degeneracy for the central caustics of close binaries. Conclusions. As far as we are aware, this is the first detection using the microlensing technique of a binary system in our Galaxy composed of an M-star and a brown dwarf. C1 [Gould, A.; Nataf, D.; Yee, J. C.; Gaudi, B. S.; Janczak, J.; Kozlowski, S.; Pogge, R. W.] Ohio State Univ, Dept Astron, Columbus, OH 43210 USA. [Albrow, M. D.; Pollard, K. R.; Hearnshaw, J. B.] Univ Canterbury, Dept Phys & Astron, Christchurch 8020, New Zealand. [Brillant, S.; Snodgrass, C.] European So Observ, Santiago 19, Chile. [Kains, N.; Bramich, D. M.] European So Observ, D-85748 Garching, Germany. [Beaulieu, J. -P.; Bertin, E.; Batista, V.; Cassan, A.; Coutures, C.; Dieters, S.; Marquette, J. -B.] Univ Paris 06, Inst Astrophys Paris, CNRS, F-75014 Paris, France. [Wambsganss, J.; Zub, M.; Liebig, C.; Maier, G.; Zimmer, F.] Heidelberg Univ, ARI, Zentrum Astron, D-69120 Heidelberg, Germany. [Horne, K.; Dominik, M.; Kains, N.; Browne, P.; Liebig, C.] Univ St Andrews, Sch Phys & Astron, Scottish Univ Phys Alliance, St Andrews KY16 9SS, Fife, Scotland. Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. [Bennett, D. P.; Caldwell, J. A. R.] Univ Texas, McDonald Observ, Ft Davis, TX 79734 USA. [Cook, K. H.] Lawrence Livermore Natl Lab, IGPP, Livermore, CA 94551 USA. [Prester, D. Dominis] Univ Rijeka, Fac Arts & Sci, Dept Phys, Rijeka 51000, Croatia. [Donatowicz, J.] Vienna Univ Technol, Dept Comp, A-1060 Vienna, Austria. [Cole, A.; Greenhill, J.] Univ Tasmania, Sch Math & Phys, Hobart, Tas 7001, Australia. [Kane, S. R.] CALTECH, NASA Exoplanet Sci Inst, Pasadena, CA 91125 USA. [Martin, R.; Williams, A.] Perth Observ, Perth, WA 6076, Australia. [Menzies, J.] S African Astron Observ, ZA-7925 Observatory, South Africa. [Sahu, K. C.] Space Telescope Sci Inst, Baltimore, MD 21218 USA. [Han, C.] Chonnam Natl Univ, Inst Basic Sci Res, Dept Phys, Chonju 361763, South Korea. [Lee, C. -U.; Park, B. -G.; Hinse, T. C.] Korea Astron & Space Sci Inst, Taejon 305348, South Korea. [Monard, L. A. G.] Bronberg Observ, Pretoria, South Africa. [Udalski, A.; Kozlowski, S.] Univ Warsaw Observ, Warsaw, Poland. Univ Concepcion, Dept Fis, Astron Grp, Concepcion, Chile. [Tristram, P. J.] Univ Cambridge, Inst Astron, Cambridge CB3 0HA, England. [Bond, I. A.; Ling, C. H.; Sweatman, W. L.] Massey Univ, Inst Informat & Math Sci, N Shore Mail Ctr, Auckland, New Zealand. [Abe, F.; Furusawa, K.; Itow, Y.; Masuda, K.; Matsubara, Y.; Miyake, N.; Sumi, T.; Suzuki, D.; Wada, K.] Osaka Univ, Dept Earth & Space Sci, Osaka 5600043, Japan. [Kerins, E.] Univ Manchester, Jodrell Bank, Ctr Astrophys, Manchester M13 9PL, Lancs, England. [Muraki, Y.] Konan Univ, Dept Phys, Kobe, Hyogo 6588501, Japan. [Ohnishi, K.] Nagano Natl Coll Technol, Nagano 3818550, Japan. [Botzler, C. S.; Rattenbury, N. J.] Univ Auckland, Dept Phys, Auckland 1142, New Zealand. [Saito, To.] Tokyo Metropolitan Coll Ind Technol, Tokyo 1160003, Japan. Nagoya Univ, Fac Sci, Dept Phys & Astrophys, Nagoya, Aichi 4648602, Japan. [Korpela, A. V.; Sullivan, D.] Mt John Observ, Lake Tekapo, New Zealand. [Tsapras, Y.; Street, R. A.; Hawkins, E.; Lister, T. A.; Saunders, E. S.] Las Cumbres Observ, Goleta, CA 93117 USA. [Bode, M. F.; Clay, N.; Fraser, S. N.; Mottram, C. J.; Steele, I. A.] Liverpool John Moores Univ, Astrophys Res Inst, Birkenhead CH41 1LD, Merseyside, England. [Allan, A.; Saunders, E. S.] Univ Exeter, Sch Phys, Exeter EX4 4QL, Devon, England. [Wheatley, P. J.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Street, R. A.] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA. [Bachelet, E.; Fouque, P.] Univ Toulouse, IRAP, CNRS, F-31400 Toulouse, France. [Jorgensen, U. G.; Mathiasen, M.; Harpsoe, K.; Hinse, T. C.; Skottfelt, J.] Univ Copenhagen, Niels Bohr Inst, DK-2100 Copenhagen, Denmark. [Jorgensen, U. G.; Mathiasen, M.; Harpsoe, K.; Hinse, T. C.; Skottfelt, J.] Univ Copenhagen, Ctr Star & Planet Format, DK-2100 Copenhagen, Denmark. Univ Observ Munich, D-81679 Munich, Germany. [Mancini, L.] Max Planck Inst Astron, D-69117 Heidelberg, Germany. [Heyrovsky, D.] Charles Univ Prague, Inst Theoret Phys, CR-18000 Prague, Czech Republic. Bellatrix Observ, I-03023 Ceccano, Italy. [Bozza, V.; Novati, S. Calchi; Scarpetta, G.] IIASS, Sez Napoli, INFN, Vietri Sur Mare, Italy. [Botzler, C. S.; Bozza, V.; Novati, S. Calchi; Scarpetta, G.] Univ Salerno, Dipartimento Fis, Fisciano, Italy. [Hinse, T. C.] Armagh Observ, Armagh BT61 9DG, North Ireland. [Rahvar, S.] Sharif Univ Technol, Dept Phys, Tehran, Iran. [Dreizler, S.; Hessman, F. V.; Hundertmark, M.] Univ Gottingen, Inst Astrophys, D-37077 Gottingen, Germany. [Finet, F.; Ricci, D.; Surdej, J.] Inst Astrophys & Geophys, B-4000 Liege, Belgium. [Southworth, J.] Univ Keele, Astrophys Grp, Newcastle Under Lyme ST5 5BG, England. Osserv Astron Brera, INAF, I-23846 Merate, LC, Italy. [Burgdorf, M. J.] Univ Stuttgart, Deutsch SOFIA Inst, D-70569 Stuttgart, Germany. [Burgdorf, M. J.] NASA, SOFIA Sci Ctr, Ames Res Ctr, Moffett Field, CA 94035 USA. Kyoto Univ, Dept Astron, Kyoto 6068502, Japan. [Tsapras, Y.] Queen Mary Univ London, Sch Math Sci, London E1 4NS, England. [Drummond, J.] Possum Observ, Patutahi, Gisbourne, New Zealand. [Maoz, D.; Kaspi, S.; Polishook, D.; Shporer, A.] Tel Aviv Univ, Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Maoz, D.; Kaspi, S.; Polishook, D.; Shporer, A.] Tel Aviv Univ, Wise Observ, IL-69978 Tel Aviv, Israel. [Christie, G. W.; Natusch, T.] Auckland Observ, Auckland, New Zealand. [McCormick, J.] Ctr Backyard Astrophys, Farm Cove Observ, Auckland, New Zealand. [Matsunaga, N.] Univ Tokyo, Inst Astron, Kiso Observ, Nagano 3970101, Japan. [Oi, N.] Grad Univ Adv Studies Sokendai, Mitaka, Tokyo 1818588, Japan. [Renon, N.] Univ Toulouse, DTSI Univ Paul Sabatier, CALMIP, F-31062 Toulouse, France. [Rahvar, S.] Perimeter Inst Theoret Phys, Waterloo, ON N2L 2Y5, Canada. [Mancini, L.] Int Inst Adv Sci Studies, I-84019 Vietri Sul Mare, SA, Italy. [Mancini, L.] Univ Salerno, Dept Phys, I-84084 Fisciano, SA, Italy. [Glitrup, M.; Grundahl, F.] Aarhus Univ, Dept Phys & Astron, DK-8000 Aarhus C, Denmark. [Bos, M.] Molehill Astron Observ, Auckland, New Zealand. [Munoz, J. A.] Univ Valencia, Dept Astron & Astrofis, E-46100 Valencia, Spain. Texas A&M Univ, Dept Phys, College Stn, TX 77843 USA. [Dong, Subo] Inst Adv Study, Princeton, NJ 08540 USA. [Natusch, T.] AUT Univ, Auckland, New Zealand. [Fukui, A.] Natl Inst Nat Sci, Natl Astron Observ Japan, Okayama Astrophys Observ, Kamogatacho, Okayama 7190232, Japan. EM gwchristie@christie.org.nz; farmcoveobs@xtra.co.nz; john_drummond@xtra.co.nz; shai@wise.tau.ac.il; shporer@wise.tau.ac.il RI Hundertmark, Markus/C-6190-2015; Rahvar, Sohrab/A-9350-2008; Kane, Stephen/B-4798-2013; Greenhill, John/C-8367-2013; Kozlowski, Szymon/G-4799-2013; Williams, Andrew/K-2931-2013; Zimmer, Fabian/M-4765-2014; Heyrovsky, David/A-2031-2015 OI Ricci, Davide/0000-0002-9790-0552; Snodgrass, Colin/0000-0001-9328-2905; Wheatley, Peter/0000-0003-1452-2240; Hundertmark, Markus/0000-0003-0961-5231; Rahvar, Sohrab/0000-0002-7084-5725; Dominik, Martin/0000-0002-3202-0343; Cole, Andrew/0000-0003-0303-3855; Kozlowski, Szymon/0000-0003-4084-880X; Williams, Andrew/0000-0001-9080-0105; Heyrovsky, David/0000-0002-5198-5343 FU French Agence Nationale de la Recherche; Czech Science Foundation [GACR 205/07/0824]; Czech Ministry of Education [MSM0021620860]; National Research Foundation of Korea [2009-0081561]; Department for Culture, Arts and Leisure, Northern Ireland, UK; Korea Research Council for Fundamental Science and Technology (KRCF); Communaute francaise de Belgique - Actions de recherche concertees - Academie universitaire Wallonie-Europe; European Community [229517]; NSF [AST-1103471, 2009068160]; NASA [NNG04GL51G]; Qatar Foundation through QNRF [NPRP-09-476-1-78]; Korea Astronomy and Space Science Institute (KASI) [2012-1-410-02]; [JSPS18253002]; [JSPS20340052]; [JSPS20740104] FX We are very grateful to the observatories that support our science (Bronberg, Canopus, CTIO, ESO, IRSF, LCOGT, Liverpool, LOAO, MOA, OGLE, Perth, SAAO, Skinakas) via the generous allocation of time that makes this work possible. The operation of Canopus Observatory is in part supported by a financial contribution from David Warren. Allocation of the Holmes grant from the French Agence Nationale de la Recherche has been indispensable to finance observing trips and travel costs for meetings, and is gratefully acknowledged here. D. H. was supported by Czech Science Foundation grant GACR 205/07/0824 and by the Czech Ministry of Education project MSM0021620860. C. H. was supported by the grant 2009-0081561 of National Research Foundation of Korea. T. C. H. was financed for his astronomical research at the Armagh Observatory by the Department for Culture, Arts and Leisure, Northern Ireland, UK and is now supported by the Korea Research Council for Fundamental Science and Technology (KRCF) via the Young Scientist Research Fellowship Program. MOA project was funded by JSPS18253002 and JSPS20340052. T. S. was funded by JSPS20740104. D. R. and J.S. acknowledge support from the Communaute francaise de Belgique - Actions de recherche concertees - Academie universitaire Wallonie-Europe. P. F. wishes to thank Noriyuki Matsunaga for discussions about the interplay between adopted distance and derived extinction. The research leading to these results has received funding from the European Community's Seventh Framework Programme (/FP7/2007-2013/) under grant agreement No 229517. A. Gould acknowledges support from NSF AST-1103471. B. S. Gaudi, A. Gould, and R. W. Pogge acknowledge support from NASA grant NNG04GL51G. Work by J. C. Yee is supported by a National Science Foundation Graduate Research Fellowship under Grant No. 2009068160. Work by S. Dong was performed under contract with the California Institute of Technology (Caltech) funded by NASA through the Sagan Fellowship Program. The RoboNet team is supported by the Qatar Foundation through QNRF grant NPRP-09-476-1-78. CUL acknowledges support by Korea Astronomy and Space Science Institute (KASI) grant 2012-1-410-02. This publication makes use of data products from the 2MASS project, as well as the SIMBAD database, Aladin and Vizier catalogue operation tools (CDS Strasbourg, France). The Two Micron All Sky Survey is a joint project of the University of Massachusetts and the Infrared Processing and Analysis Center/California Institute of Technology, funded by the National Aeronautics and Space Administration and the National Science Foundation. This work was granted access to the HPC resources of CALMIP under the allocation 2012-[1131]. NR 57 TC 10 Z9 10 U1 1 U2 14 PU EDP SCIENCES S A PI LES ULIS CEDEX A PA 17, AVE DU HOGGAR, PA COURTABOEUF, BP 112, F-91944 LES ULIS CEDEX A, FRANCE SN 0004-6361 EI 1432-0746 J9 ASTRON ASTROPHYS JI Astron. Astrophys. PD NOV PY 2012 VL 547 AR A55 DI 10.1051/0004-6361/201219765 PG 12 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 036MZ UT WOS:000311031700055 ER PT J AU in 't Zand, JJM Homan, J Keek, L Palmer, DM AF in 't Zand, J. J. M. Homan, J. Keek, L. Palmer, D. M. TI Superexpansion as a possible probe of accretion in 4U 1820-30 SO ASTRONOMY & ASTROPHYSICS LA English DT Article DE accretion, accretion disks; X-rays: binaries; X-rays: bursts; stars: neutron; X-rays: individuals: 4U 1820-30 ID X-RAY-BURSTS; PHOTOSPHERIC RADIUS EXPANSION; CLUSTER NGC 6624; NEUTRON-STARS; THERMONUCLEAR BURST; TIMING-EXPLORER; SUPERORBITAL VARIABILITY; IGR J17473-2721; TERZAN 5; OSCILLATIONS AB The ultracompact X-ray binary 4U 1820-30 is well known for its approximate to 170-d superorbital modulation in X-ray flux and spectrum, and the exclusiveness of bursting behavior to the low hard "island" state. In May-June 2009, there was an exceptionally long 51-d low state. This state was well covered by X-ray observations and 12 bursts were detected, 9 with the high-throughput RXTE. We investigate the character of these X-ray bursts and find an interesting change in their photospheric expansion behavior. At the lowest inferred mass accretion rates, this expansion becomes very large in 4 bursts and reaches the so-called superexpansion regime. We speculate that this is due to the geometry of the inner accretion flow being spherical and a decreasing accretion rate: when the flow geometry nearest to the neutron star is spherical and the accretion rate is low, the ram pressure of the accretion disk may become too low to counteract that of the photospheric expansion. In effect, this may provide a novel means to probe the accretion flow. Additionally, we observe a peculiar effect: the well-known cessation of X-ray bursts in the high state is too quick to be consistent with a transition to stable helium burning. We suggest an alternative explanation, that the cessation is due to the introduction of a non-nuclear heat source in the neutron star ocean. C1 [in 't Zand, J. J. M.] SRON Netherlands Inst Space Res, NL-3584 CA Utrecht, Netherlands. [Homan, J.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Homan, J.] MIT, Kavli Inst Astrophys & Space Res, Cambridge, MA 02139 USA. [Keek, L.] Michigan State Univ, Natl Superconducting Cyclotron Lab, Dept Phys & Astron, E Lansing, MI 48824 USA. [Keek, L.] Michigan State Univ, Joint Inst Nucl Astrophys, E Lansing, MI 48824 USA. [Palmer, D. M.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP in 't Zand, JJM (reprint author), SRON Netherlands Inst Space Res, Sorbonnelaan 2, NL-3584 CA Utrecht, Netherlands. EM jeanz@sron.nl FU International Space Science Institute (ISSI) in Bern; Joint Institute for Nuclear Astrophysics (JINA), a National Science Foundation Physics Frontier Center [PHY08-22648] FX We thank Nevin Weinberg (MIT), Ed Brown (MSU) and Tullio Bagnoli (SRON) for useful discussions. J.Z. and L. K. are members of an International Team in Space Science on type-I X-ray bursts sponsored by the International Space Science Institute (ISSI) in Bern and thank ISSI for the hospitality during part of this work. We are grateful to the anonymous referee for constructive comments that helped improve the paper. L. K. is supported by the Joint Institute for Nuclear Astrophysics (JINA; grant PHY08-22648), a National Science Foundation Physics Frontier Center. This paper utilizes data from the Multi-INstrument Burst ARchive (MINBAR). RXTE/ASM and Swift/BAT results were provided by the RXTE/ASM and Swift/BAT team, respectively. NR 60 TC 10 Z9 10 U1 0 U2 0 PU EDP SCIENCES S A PI LES ULIS CEDEX A PA 17, AVE DU HOGGAR, PA COURTABOEUF, BP 112, F-91944 LES ULIS CEDEX A, FRANCE SN 0004-6361 J9 ASTRON ASTROPHYS JI Astron. Astrophys. PD NOV PY 2012 VL 547 AR A47 DI 10.1051/0004-6361/201220141 PG 8 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 036MZ UT WOS:000311031700047 ER PT J AU Noterdaeme, P Petitjean, P Carithers, WC Paris, I Font-Ribera, A Bailey, S Aubourg, E Bizyaev, D Ebelke, G Finley, H Ge, J Malanushenko, E Malanushenko, V Miralda-Escude, J Myers, AD Oravetz, D Pan, K Pieri, MM Ross, NP Schneider, DP Simmons, A York, DG AF Noterdaeme, P. Petitjean, P. Carithers, W. C. Paris, I. Font-Ribera, A. Bailey, S. Aubourg, E. Bizyaev, D. Ebelke, G. Finley, H. Ge, J. Malanushenko, E. Malanushenko, V. Miralda-Escude, J. Myers, A. D. Oravetz, D. Pan, K. Pieri, M. M. Ross, N. P. Schneider, D. P. Simmons, A. York, D. G. TI Column density distribution and cosmological mass density of neutral gas: Sloan Digital Sky Survey-III Data Release 9 SO ASTRONOMY & ASTROPHYSICS LA English DT Article DE cosmology: observations; quasars: absorption lines; galaxies: evolution ID LY-ALPHA SYSTEMS; SDSS-III; SPECTROSCOPIC SURVEY; TARGET SELECTION; GALAXIES; ABSORPTION; TELESCOPE; EVOLUTION AB We present the first results from an ongoing survey for damped Lyman-alpha systems (DLAs) in the spectra of z > 2 quasars observed in the course of the Baryon Oscillation Spectroscopic Survey (BOSS), which is part of the Sloan Digital Sky Survey (SDSS) III. Our full (non-statistical) sample, based on Data Release 9, comprises 12 081 systems with log N(H I) >= 20, out of which 6839 have log N(H I) >= 20.3. This is the largest DLA sample ever compiled, superseding that from SDSS-II by a factor of seven. Using a statistical sub-sample and estimating systematics from realistic mock data, we probe the N(H I) distribution at < z > = 2.5. Contrary to what is generally believed, the distribution extends beyond 10(22) cm(-2) with a moderate slope of index approximate to-3.5. This result matches the opacity-corrected distribution observed at z = 0 surprisingly well. The cosmological mass density of neutral gas in DLAs is found to be Omega(DLA)(g) approximate to 10(-3), evolving only mildly over the past 12 billion years. C1 [Noterdaeme, P.; Petitjean, P.; Finley, H.] CNRS UPMC, Inst Astrophys Paris, UMR 7095, F-75014 Paris, France. [Carithers, W. C.; Font-Ribera, A.; Bailey, S.; Ross, N. P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Paris, I.] Univ Chile, Dept Astron, Santiago, Chile. [Font-Ribera, A.] Univ Zurich, Inst Theoret Phys, CH-8057 Zurich, Switzerland. [Aubourg, E.] CNRS UMR 7164, APC, F-75205 Paris 13, France. [Bizyaev, D.; Ebelke, G.; Malanushenko, E.; Malanushenko, V.; Oravetz, D.; Pan, K.; Simmons, A.] Apache Point Observ, Sunspot, NM 88349 USA. [Ge, J.] Univ Florida, Dept Astron, Bryant Space Sci Ctr 211, Gainesville, FL 32611 USA. [Miralda-Escude, J.] Univ Barcelona, Fac Fis, Inst Ciencies Cosmos, E-08028 Barcelona, Spain. [Myers, A. D.] Univ Wyoming, Dept Phys & Astron, Laramie, WY 82071 USA. [Pieri, M. M.] Univ Portsmouth, Inst Cosmol & Gravitat, Portsmouth PO1 2UP, Hants, England. [Schneider, D. P.] Penn State Univ, Dept Astron & Astrophys, University Pk, PA 16802 USA. [Schneider, D. P.] Penn State Univ, Inst Gravitat & Cosmos, University Pk, PA 16802 USA. [York, D. G.] Univ Chicago, Dept Astron & Astrophys, Chicago, IL 60637 USA. [York, D. G.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. RP Noterdaeme, P (reprint author), CNRS UPMC, Inst Astrophys Paris, UMR 7095, 98Bis Bd Arago, F-75014 Paris, France. EM noterdaeme@iap.fr OI Miralda-Escude, Jordi/0000-0002-2316-8370; Finley, Hayley/0000-0002-1216-8914 FU Agence Nationale de la Recherche [ANR-08-BLAN-0222]; Alfred P. Sloan Foundation; National Science Foundation; US Department of Energy Office of Science; University of Arizona; Brazilian Participation Group; Brookhaven National Laboratory; University of Cambridge; Carnegie Mellon University; University of Florida; French Participation Group; German Participation Group; Harvard University; Instituto de Astrofisica de Canarias; Michigan State/Notre Dame/JINA Participation Group; Johns Hopkins University; Lawrence Berkeley National Laboratory; Max Planck Institute for Astrophysics; Max Planck Institute for Extraterrestrial Physics; New Mexico State University; New York University; Ohio State University; Pennsylvania State University; University of Portsmouth; Princeton University; Spanish Participation Group; University of Tokyo; University of Utah; Vanderbilt University; University of Virginia; University of Washington; Yale University FX We thank the anonymous referee for helpful comments and suggestions. The French participation group to SDSS-III was supported by the Agence Nationale de la Recherche under grant ANR-08-BLAN-0222. Funding for SDSS-III has been provided by the Alfred P. Sloan Foundation, the Participating Institutions, the National Science Foundation, and the US Department of Energy Office of Science. The SDSS-III web site is http://www.sdss3.org/. SDSS-III is managed by the Astrophysical Research Consortium for the Participating Institutions of the SDSS-III Collaboration including the University of Arizona, the Brazilian Participation Group, Brookhaven National Laboratory, University of Cambridge, Carnegie Mellon University, University of Florida, the French Participation Group, the German Participation Group, Harvard University, the Instituto de Astrofisica de Canarias, the Michigan State/Notre Dame/JINA Participation Group, Johns Hopkins University, Lawrence Berkeley National Laboratory, Max Planck Institute for Astrophysics, Max Planck Institute for Extraterrestrial Physics, New Mexico State University, New York University, Ohio State University, Pennsylvania State University, University of Portsmouth, Princeton University, the Spanish Participation Group, University of Tokyo, University of Utah, Vanderbilt University, University of Virginia, University of Washington, and Yale University. NR 32 TC 87 Z9 88 U1 1 U2 3 PU EDP SCIENCES S A PI LES ULIS CEDEX A PA 17, AVE DU HOGGAR, PA COURTABOEUF, BP 112, F-91944 LES ULIS CEDEX A, FRANCE SN 0004-6361 J9 ASTRON ASTROPHYS JI Astron. Astrophys. PD NOV PY 2012 VL 547 AR L1 DI 10.1051/0004-6361/201220259 PG 4 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 036MZ UT WOS:000311031700123 ER PT J AU Selig, MJ Hsieh, CWC Thygesen, LG Himmel, ME Felby, C Decker, SR AF Selig, Michael J. Hsieh, Chia-Wen Carmen Thygesen, Lisbeth G. Himmel, Michael E. Felby, Claus Decker, Stephen R. TI Considering water availability and the effect of solute concentration on high solids saccharification of lignocellulosic biomass SO BIOTECHNOLOGY PROGRESS LA English DT Article DE high solids; water activity; cellulose; lignocellulose; saccharification ID ENZYMATIC-HYDROLYSIS; CORN STOVER AB Milliliter scale (ligno)cellulose saccharifications suggest general solute concentration and its impact on water availability plays a significant role in detrimental effects associated with high solids lignocellulose conversions. A microtumbler developed to enable free-fall mixing at dry solids loadings up to 35% (w/w) repeatedly produced known detrimental conversion trends on cellulose, xylan and pretreated lignocellulose with commercial enzymes. Despite this, high concentrations of insoluble nonhydrolysable dextrans did not depress saccharification extents in 5% (w/w) cellulose slurries suggesting mass transfer limitations may not significantly limit hydrolysis extents at high solids loadings. Interestingly, cellulose saccharification by purified cellulases showed increased conversions with increasing dry solids loadings. This prompted investigations into impacts the concentration of soluble species, such as sugar alcohols, low molecular weight enzyme preparation components, and monomer hydrolysis products, have on the hydrolysis environment. Such substances significantly depress conversion rates and were shown to correlatively lower water activity (Aw) in the hydrolysis environment while high insoluble solids concentrations did not. Furthermore, low-field NMR on concentrated slurries of insoluble complex carbohydrates, including the nonhydrolysable dextrans, showed all solids constrained water significantly more than high concentrations of soluble species (inhibitory) suggesting water constraint may not be as problematic an issue at high solids loadings compared to the availability of water in the system. Additionally, the introduction of soluble species lessened overall water constraint in high solids systems and appears to shift the distribution of water away from insoluble surfaces. This is potentially a critical issue for industrial processes operating at high dry solids levels. (C) 2012 American Institute of Chemical Engineers Biotechnol. Prog., 2012 C1 [Selig, Michael J.; Hsieh, Chia-Wen Carmen; Thygesen, Lisbeth G.; Felby, Claus] Univ Copenhagen, Fac Life Sci, Frederiksberg, Denmark. [Himmel, Michael E.; Decker, Stephen R.] Natl Renewable Energy Lab, Biosci Ctr, Golden, CO USA. RP Selig, MJ (reprint author), Univ Copenhagen, Fac Life Sci, Frederiksberg, Denmark. EM mjs@life.ku.dk OI Thygesen, Lisbeth Garbrecht/0000-0001-9685-7460; Felby, Claus/0000-0002-6537-0155 NR 17 TC 27 Z9 27 U1 1 U2 69 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 8756-7938 J9 BIOTECHNOL PROGR JI Biotechnol. Prog. PD NOV-DEC PY 2012 VL 28 IS 6 BP 1478 EP 1490 DI 10.1002/btpr.1617 PG 13 WC Biotechnology & Applied Microbiology; Food Science & Technology SC Biotechnology & Applied Microbiology; Food Science & Technology GA 051VX UT WOS:000312157100012 PM 22915470 ER PT J AU Robertson, BA Rice, RA Sillett, TS Ribic, CA Babcock, BA Landis, DA Herkert, JR Fletcher, RJ Fontaine, JJ Doran, PJ Schemske, DW AF Robertson, Bruce A. Rice, Robert A. Sillett, T. Scott Ribic, Christine A. Babcock, Bruce A. Landis, Douglas A. Herkert, James R. Fletcher, Robert J., Jr. Fontaine, Joseph J. Doran, Patrick J. Schemske, Douglas W. TI ARE AGROFUELS A CONSERVATION THREAT OR OPPORTUNITY FOR GRASSLAND BIRDS IN THE UNITED STATES? SO CONDOR LA English DT Review DE biofuels; biodiversity; cellulosic ethanol; Conservation Reserve Program; prairie; switchgrass ID REED CANARY-GRASS; RESERVE PROGRAM; BIOMASS ENERGY; AGRICULTURAL LANDSCAPES; HARVESTING SWITCHGRASS; FARMLAND BIODIVERSITY; PHALARIS-ARUNDINACEA; SPECIES-DIVERSITY; AREA SENSITIVITY; BREEDING BIRDS AB In the United States, government-mandated growth in the production of crops dedicated to bionic! (agrofuels) is predicted to increase the demands on existing agricultural lands, potentially threatening the persistence of populations of grassland birds they support. We review recently published literature and datasets to ( 1) examine the ability of alternative agrofuel crops and their management regimes to provide habitat for grassland birds, (2) determine how crop placement in agricultural landscapes and agrofuel-related land-use change will affect grassland birds, and (3) identify critical research and policy-development needs associated with agrofuel production. We find that native perennial plants proposed as feedstock for agrofuel (switchgrass, Panicum virgatum, and mixed grass-forb prairie) have considerable potential to provide new habitat to a wide range of grassland birds, including rare and threatened species. However, industrialization of agrofuel production that maximizes biomass, homogenizes vegetation structure, and results in the cultivation of small fields within largely forested landscapes is likely to reduce species richness and/or abundance of grassland-dependent birds. Realizing the potential benefits of agrofuel production for grassland birds' conservation will require the development of new policies that encourage agricultural practices specifically targeting the needs of grassland specialists. The broad array of grower-incentive programs in existence may deliver new agrofuel policies effectively but will require coordination at a spatial scale broader than currently practiced, preferably within an adaptive-management framework. C1 [Robertson, Bruce A.; Rice, Robert A.; Sillett, T. Scott] Smithsonian Conservat Biol Inst, Migratory Bird Ctr, Washington, DC 20008 USA. [Robertson, Bruce A.; Landis, Douglas A.; Schemske, Douglas W.] Michigan State Univ, DOE Great Lakes Bioenergy Res Ctr, E Lansing, MI 48824 USA. [Robertson, Bruce A.] Bard Coll, Div Sci Math & Comp, Annandale On Hudson, NY 12504 USA. [Ribic, Christine A.] Univ Wisconsin, US Geol Survey, Wisconsin Cooperat Wildlife Res Unit, Madison, WI 53706 USA. [Babcock, Bruce A.] Iowa State Univ, Ctr Agr & Rural Dev, Ames, IA 50011 USA. [Landis, Douglas A.] Michigan State Univ, Dept Entomol, E Lansing, MI 48824 USA. [Herkert, James R.] Univ Illinois, Illinois Nat Hist Survey, Champaign, IL 61820 USA. [Fletcher, Robert J., Jr.] Univ Florida, Dept Wildlife Ecol & Conservat, Gainesville, FL 32611 USA. [Fontaine, Joseph J.] Univ Nebraska, US Geol Survey, Nebraska Cooperat Fish & Wildlife Res Unit, Sch Nat Resources, Lincoln, NE 68583 USA. [Doran, Patrick J.] Nature Conservancy, Lansing, MI 48906 USA. RP Robertson, BA (reprint author), Smithsonian Conservat Biol Inst, Migratory Bird Ctr, Natl Zool Pk, Washington, DC 20008 USA. EM broberts@bard.edu RI Fontaine, Joseph/F-6557-2010; OI Fontaine, Joseph/0000-0002-7639-9156; Fletcher, Robert/0000-0003-1717-5707 FU DOE Office of Science [DE-FC02-07ER64494]; Office of Energy Efficiency and Renewable Energy [DE-AC05-76RL01830]; U.S. National Science Foundation LTER program [DEB 1027253]; MSU AgBioResearch; U.S. Fish and Wildlife Service; Migratory Bird Joint Ventures Midwest Region [30181AG045]; Smithsonian Conservation Biology Institute; Nature Conservancy's Great Lakes Fund FX Financial support for this work was provided by the DOE Office of Science (DE-FC02-07ER64494) and Office of Energy Efficiency and Renewable Energy (DE-AC05-76RL01830), the U.S. National Science Foundation LTER program (DEB 1027253), MSU AgBioResearch, U.S. Fish and Wildlife Service, Migratory Bird Joint Ventures Midwest Region grant 30181AG045. Bruce Robertson was supported by a fellowship from the Smithsonian Conservation Biology Institute. Patrick Doran was supported by The Nature Conservancy's Great Lakes Fund for Partnership in Conservation Science and Economics. NR 75 TC 14 Z9 14 U1 0 U2 58 PU COOPER ORNITHOLOGICAL SOC PI LAWRENCE PA ORNITHOLOGICAL SOC NORTH AMER PO BOX 1897, LAWRENCE, KS 66044-8897 USA SN 0010-5422 J9 CONDOR JI Condor PD NOV PY 2012 VL 114 IS 4 BP 679 EP 688 DI 10.1525/cond.2012.110136 PG 10 WC Ornithology SC Zoology GA 048AN UT WOS:000311882700001 ER PT J AU Li, CP Lin, F Richards, RM Engtrakul, C Dillon, AC Tenent, RC Wolden, CA AF Li, Chi-Ping Lin, Feng Richards, Ryan M. Engtrakul, Chaiwat Dillon, Anne C. Tenent, Robert C. Wolden, Colin A. TI Ultrasonic spray deposition of high performance WO3 films using template-assisted sol-gel chemistry SO ELECTROCHEMISTRY COMMUNICATIONS LA English DT Article DE Tungsten oxide; Electrochromics; Ultrasonic spray deposition; Mesoporous; Sol-gel ID TUNGSTEN-OXIDE; THIN-FILMS; SILICA AB Tungsten oxide (WO3) thin films with nanoscale porosity were prepared by adopting templating sol-gel chemistry to ultrasonic spray deposition (USD). It was found that the electrochromic performance was strongly correlated to the annealing conditions used to remove the triblock copolymer template. Optimized films display state-of-the-art performance with respect to coloration efficiency (>50 cm(2)/C). optical modulation (>75%), and switching times (<10 s). The films exhibit good durability, displaying disordered, nanocrystalline morphology. USD is compatible with in line manufacturing, and the performance was notably improved over films deposited by spin coating using the same chemistry. (C) 2012 Elsevier B.V. All rights reserved. C1 [Li, Chi-Ping; Lin, Feng; Richards, Ryan M.; Wolden, Colin A.] Colorado Sch Mines, Mat Sci Program, Golden, CO 80401 USA. [Li, Chi-Ping; Lin, Feng; Engtrakul, Chaiwat; Dillon, Anne C.; Tenent, Robert C.] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Wolden, CA (reprint author), Colorado Sch Mines, Mat Sci Program, Golden, CO 80401 USA. EM cwolden@mines.edu RI Lin, Feng/H-5027-2012; Engtrakul, Chaiwat/H-5634-2011; Richards, Ryan/B-3513-2008 OI Lin, Feng/0000-0001-7286-7525; FU National Science Foundation [DMR-0820518]; Department of Energy [DE-AC36-08GO28308] FX This research was founded by the National Science Foundation through award DMR-0820518 and the Department of Energy under subcontract DE-AC36-08GO28308. We gratefully thank Dr. Rachel Morrish for assistance with Raman spectroscopy and Dr. Mayur Ostwal for performing the physisorption measurements. NR 17 TC 10 Z9 10 U1 0 U2 57 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 1388-2481 J9 ELECTROCHEM COMMUN JI Electrochem. Commun. PD NOV PY 2012 VL 25 BP 62 EP 65 DI 10.1016/j.elecom.2012.09.017 PG 4 WC Electrochemistry SC Electrochemistry GA 048QJ UT WOS:000311927300017 ER PT J AU You, H Pierce, M Komanicky, V Barbour, A Zhu, CH AF You, Hoydoo Pierce, Michael Komanicky, Vladimir Barbour, Andi Zhu, Chenhui TI Study of electrode surface dynamics using coherent surface X-ray scattering SO ELECTROCHIMICA ACTA LA English DT Article; Proceedings Paper CT 62nd Annual Meeting of the International-Society-of-Electrochemistry CY SEP 11-15, 2011 CL Niigata, JAPAN DE Surface reconstruction; Coherent X-ray scattering; Surface X-ray scattering; Surface dynamics; X-ray speckles ID SCANNING-TUNNELING-MICROSCOPY; POTENTIAL-INDUCED RECONSTRUCTION; REFLECTIVITY; DIFFRACTION; AU(100); INTERFACE; BEHAVIOR; AU(001); AU(111) AB We present a coherent X-ray scattering technique that allows in situ measurements of electrode surface dynamics. This technique can measure the transient dynamics of phase relaxation from one phase to another upon changing electrochemical conditions or temperature. It can also measure the dynamics of microstates even if the electrode is apparently static in macroscopic states. We will discuss the underlying physics of the X-ray speckle correlation spectroscopy and present our recent study of Au (1 0 0) surface in vacuum, water, and electrolytes. (C) 2012 Elsevier Ltd. All rights reserved. C1 [You, Hoydoo; Pierce, Michael; Komanicky, Vladimir; Barbour, Andi; Zhu, Chenhui] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Pierce, Michael] Rochester Inst Technol, Dept Phys, Rochester, NY 14623 USA. [Komanicky, Vladimir] Safarik Univ, Fac Sci, Kosice 04154, Slovakia. RP You, H (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM hyou@anl.gov RI Pierce, Michael/D-5570-2014; You, Hoydoo/A-6201-2011 OI Pierce, Michael/0000-0002-9209-8556; You, Hoydoo/0000-0003-2996-9483 FU U.S. Department of Energy, Office of Basic Energy Sciences, Materials Science Division; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-06CH11357]; Slovak grant VEGA [1/0782/12] FX This work was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Materials Science Division and the use of the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Basic Energy Sciences under Contract No. DE-AC02-06CH11357. The work at Safarik University was supported by Slovak grant VEGA 1/0782/12. We thank A. Sandy and J.-D. Su for their assistance during the experiments. NR 32 TC 2 Z9 2 U1 3 U2 22 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0013-4686 EI 1873-3859 J9 ELECTROCHIM ACTA JI Electrochim. Acta PD NOV 1 PY 2012 VL 82 SI SI BP 570 EP 575 DI 10.1016/j.electacta.2012.03.069 PG 6 WC Electrochemistry SC Electrochemistry GA 047XC UT WOS:000311873800079 ER PT J AU Crandall, RS Iwaniczko, E Li, JV Page, MR AF Crandall, Richard S. Iwaniczko, Eugene Li, Jian V. Page, Mathew R. TI A comprehensive study of hole collection in heterojunction solar cells SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID HYDROGENATED AMORPHOUS-SILICON; BAND OFFSETS; INTERNAL PHOTOEMISSION; SI-H; TRANSPORT; THERMODYNAMICS; MECHANISMS; DEFECTS; ENTROPY AB We conduct a systematic investigation into the mechanism of hole collection in amorphous/crystalline silicon heterojunctions solar cells using transient-capacitance techniques. The devices are formed by depositing undoped amorphous silicon (i layer) followed by p-type amorphous silicon on n-type crystalline silicon wafers. For i layers varying from 3.2 to 96 nm, we find only a factor of four change in hole collection-rate at low temperature where thermal emission over the valence band offset is precluded. We conclude that holes traverse the i layer by hopping through defects rather than direct tunneling through the entire i layer. This process is weakly thermally activated with a rate above 1 x 10(4) s(-1) at room temperature. Near room temperature and with thick i layers, we observe hole collection with a high activation energy that depends on measurement conditions. We demonstrate that hopping through defects is the dominant mode of hole collection for solar cell operation at room temperature and above. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4764031] C1 [Crandall, Richard S.; Iwaniczko, Eugene; Li, Jian V.; Page, Mathew R.] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Crandall, RS (reprint author), Natl Renewable Energy Lab, 15013 Denver W Pkwy, Golden, CO 80401 USA. RI Li, Jian/B-1627-2016 FU U.S. Department of Energy [DE-AC36-08GO28308] FX We gratefully acknowledge support from the U.S. Department of Energy under Contract No. DE-AC36-08GO28308. The authors thank Ana Kanevce for helpful discussions and sharing results of simulations. This paper is dedicated to the memory of Eugene Iwaniczko. NR 27 TC 8 Z9 8 U1 2 U2 31 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 J9 J APPL PHYS JI J. Appl. Phys. PD NOV 1 PY 2012 VL 112 IS 9 AR 093713 DI 10.1063/1.4764031 PG 9 WC Physics, Applied SC Physics GA 049FS UT WOS:000311968400060 ER PT J AU Dongmo, P Zhong, YJ Attia, P Bomberger, C Cheaito, R Ihlefeld, JF Hopkins, PE Zide, J AF Dongmo, Pernell Zhong, Yujun Attia, Peter Bomberger, Cory Cheaito, Ramez Ihlefeld, Jon F. Hopkins, Patrick E. Zide, Joshua TI Enhanced room temperature electronic and thermoelectric properties of the dilute bismuthide InGaBiAs SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID MULTILAYER THERMIONIC REFRIGERATION; MOLECULAR-BEAM EPITAXY; DEVICES; EFFICIENCY; TRANSPORT; GROWTH; MERIT AB We report room temperature electronic and thermoelectric properties of Si-doped In0.52Ga0.48BiyAs1-y with varying Bi concentrations. These films were grown epitaxially on a semi-insulating InP substrate by molecular beam epitaxy. We show that low Bi concentrations are optimal in improving the conductivity, Seebeck coefficient, and thermoelectric power factor, possibly due to the surfactant effects of bismuth. We observed a reduction in thermal conductivity with increasing Bi concentration, which is expected because of alloy scattering. We report a peak ZT of 0.23 at 300 K. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4761996] C1 [Dongmo, Pernell; Zhong, Yujun; Bomberger, Cory; Zide, Joshua] Univ Delaware, Dept Mat Sci & Engn, Newark, DE 19716 USA. [Attia, Peter] Univ Delaware, Dept Chem Engn, Newark, DE 19716 USA. [Cheaito, Ramez; Hopkins, Patrick E.] Univ Virginia, Dept Mech & Aerosp Engn, Charlottesville, VA USA. [Ihlefeld, Jon F.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Dongmo, P (reprint author), Univ Delaware, Dept Mat Sci & Engn, Newark, DE 19716 USA. EM zide@udel.edu RI Ihlefeld, Jon/B-3117-2009; Zide, Joshua/B-5105-2010 OI Zide, Joshua/0000-0002-6378-7221 FU Office of Naval Research through the Young Investigator Program FX The authors would like to acknowledge the financial support of the Office of Naval Research through the Young Investigator Program. NR 32 TC 11 Z9 11 U1 0 U2 23 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 J9 J APPL PHYS JI J. Appl. Phys. PD NOV 1 PY 2012 VL 112 IS 9 AR 093710 DI 10.1063/1.4761996 PG 4 WC Physics, Applied SC Physics GA 049FS UT WOS:000311968400057 ER PT J AU Duda, JC Kimmer, CJ Soffa, WA Zhou, XW Jones, RE Hopkins, PE AF Duda, J. C. Kimmer, C. J. Soffa, W. A. Zhou, X. W. Jones, R. E. Hopkins, P. E. TI Influence of crystallographic orientation and anisotropy on Kapitza conductance via classical molecular dynamics simulations SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID THERMAL-BOUNDARY CONDUCTANCE; CONDUCTIVITY; SUPERLATTICES; INTERFACES; TRANSPORT AB We investigate the influence of crystallographic orientation and anisotropy on local phonon density of states, phonon transmissivity, and Kapitza conductance at interfaces between Lennard-Jones solids via classical molecular dynamics simulations. In agreement with prior works, we find that the Kapitza conductance at an interface between two face-centered cubic materials is independent of crystallographic orientation. On the other hand, at an interface between a face-centered cubic material and a tetragonal material, the Kapitza conductance is strongly dependent on the relative orientation of the tetragonal material, albeit this dependence is subject to the overlap in vibrational spectra of the cubic and tetragonal materials. Furthermore, we show that interactions between acoustic phonons in the cubic material and optical phonons in the tetragonal material can lead to the interface exhibiting greater "thermal anisotropy" as compared to that of the constituent materials. Finally, it is noted that the relative match or mismatch between the Debye temperatures of two materials comprising an interface does not serve an accurate gauge of the efficiency of interfacial thermal transport when those materials have different crystal structures. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4764921] C1 [Duda, J. C.; Hopkins, P. E.] Univ Virginia, Dept Mech & Aerosp Engn, Charlottesville, VA 22904 USA. [Duda, J. C.] Sandia Natl Labs, Microscale Sci & Technol Dept, Albuquerque, NM 87185 USA. [Kimmer, C. J.] Indiana Univ SE, Sch Nat Sci, New Albany, IN 47150 USA. [Soffa, W. A.] Univ Virginia, Dept Mat Sci & Engn, Charlottesville, VA 22904 USA. [Zhou, X. W.; Jones, R. E.] Sandia Natl Labs, Mech Mat Dept, Livermore, CA 94550 USA. RP Duda, JC (reprint author), Univ Virginia, Dept Mech & Aerosp Engn, Charlottesville, VA 22904 USA. EM duda@virginia.edu; phopkins@virginia.edu RI Duda, John/A-7214-2011 FU LDRD program office at Sandia National Laboratories; United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors acknowledge funding through the LDRD program office at Sandia National Laboratories. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the United States Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 44 TC 10 Z9 10 U1 0 U2 24 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD NOV 1 PY 2012 VL 112 IS 9 AR 093515 DI 10.1063/1.4764921 PG 8 WC Physics, Applied SC Physics GA 049FS UT WOS:000311968400036 ER PT J AU Gupta, G Thorp, JC Mara, NA Dattelbaum, AM Misra, A Picraux, ST AF Gupta, G. Thorp, J. C. Mara, N. A. Dattelbaum, A. M. Misra, A. Picraux, S. T. TI Morphology and porosity of nanoporous Au thin films formed by dealloying of AuxSi1-x SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID GOLD; AG; FABRICATION; ELECTRODES; EVOLUTION AB We have investigated the morphology, structure, and annealing response of nanoporous Au films synthesized via electrochemical dealloying of amorphous AuxSi1-x co-deposited films on Si substrates. The starting Au alloy film concentrations were varied from x = 0.09 to 0.41 and the resulting nanoscale porous films were characterized by electron microscopy and Rutherford backscattering techniques. Our observations provide a systematic description of the nanoporous Au film morphology, porosity, and degree of collapse as a function of starting AuxSi1-x alloy composition. The characteristic pore sizes increased from 10 to 45 nm and the porosity increased from 45% to 70% for the nanoporous Au films with decrease in the starting Au concentrations. The degree of film collapse due to dealloying also increased with decreasing Au concentration. The electrochemical dealloying process for nanoporous film formation was observed to change from a layer-by-layer dealloying process to a localized, percolation-dominated process as the Au concentration was decreased from 40 to 9 at. %. The thin film porous synthesis approach presented here enables the integration of "bottom up" dealloying self-assembly with "top down" microelectronics-based fabrication techniques, making it a useful new approach for Si-based microsystem applications. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4764906] C1 [Gupta, G.; Mara, N. A.; Dattelbaum, A. M.; Misra, A.; Picraux, S. T.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. [Thorp, J. C.] Arizona State Univ, Dept Chem & Mat Engn, Tempe, AZ 85287 USA. RP Picraux, ST (reprint author), Los Alamos Natl Lab, Ctr Integrated Nanotechnol, POB 1663, Los Alamos, NM 87545 USA. EM picraux@lanl.gov RI Mara, Nathan/J-4509-2014 FU U.S. Department of Energy [DE-AC52-06NA25396] FX Work at Los Alamos National Laboratory (LANL) was performed under the auspices of the U.S. Department of Energy under Contract No. DE-AC52-06NA25396. The research was performed, in part, at the Center for Integrated Nanotechnologies (CINT), a U.S. Department of Energy, Office of Basic Energy Sciences user facility. We gratefully acknowledge insightful technical discussions with Karl Sieradzki and Lei Tang at Arizona State University and Hongqi Li at LANL. NR 26 TC 8 Z9 8 U1 1 U2 60 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD NOV 1 PY 2012 VL 112 IS 9 AR 094320 DI 10.1063/1.4764906 PG 7 WC Physics, Applied SC Physics GA 049FS UT WOS:000311968400114 ER PT J AU Liu, HR Chen, SY Zhai, YT Xiang, HJ Gong, XG Wei, SH AF Liu, Heng-Rui Chen, Shiyou Zhai, Ying-Teng Xiang, H. J. Gong, X. G. Wei, Su-Huai TI First-principles study on the effective masses of zinc-blend-derived Cu2Zn-IV-VI4 (IV = Sn, Ge, Si and VI = S, Se) SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID OPTICAL-PROPERTIES; NANOCRYSTALS; EFFICIENCY; ALLOYS; ENERGY AB The electron and hole effective masses of kesterite (KS) and stannite (ST) structured Cu2Zn-IV-VI4 (IV = Sn, Ge, Si and VI = S, Se) semiconductors are systematically studied using first-principles calculations. We find that the electron effective masses are almost isotropic, while strong anisotropies are observed for the hole effective masses. The electron effective masses are typically much smaller than the hole effective masses for all studied compounds. The ordering of the topmost three valence bands and the corresponding hole effective masses of the KS and ST structures are different due to the different sign of the crystal-field splitting. The electron and hole effective masses of Se-based compounds are significantly smaller compared to the corresponding S-based compounds. They also decrease as the atomic number of the group IV elements (Si, Ge, Sn) increases, but the decrease is less notable than that caused by the substitution of S by Se. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4759322] C1 [Liu, Heng-Rui; Zhai, Ying-Teng; Xiang, H. J.; Gong, X. G.] Fudan Univ, State Key Lab Surface Phys, Key Lab Computat Phys Sci MOE, Shanghai 200433, Peoples R China. [Liu, Heng-Rui; Zhai, Ying-Teng; Xiang, H. J.; Gong, X. G.] Fudan Univ, Dept Phys, Shanghai 200433, Peoples R China. [Chen, Shiyou] E China Normal Univ, Key Lab Polar Mat & Devices MOE, Shanghai 200241, Peoples R China. [Wei, Su-Huai] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Liu, HR (reprint author), Fudan Univ, State Key Lab Surface Phys, Key Lab Computat Phys Sci MOE, Shanghai 200433, Peoples R China. RI Xiang, Hongjun/I-4305-2016; gong, xingao/D-6532-2011 OI Xiang, Hongjun/0000-0002-9396-3214; FU Special Funds for Major State Basic Research; National Science Foundation of China; Ministry of Education; Shanghai Municipality; U.S. Department of Energy [DE-AC36-08GO28308] FX This work was partially supported by the Special Funds for Major State Basic Research, National Science Foundation of China, Ministry of Education, and Shanghai Municipality. The calculations were performed in the Supercomputer Center of Fudan University. The work at NREL was funded by the U.S. Department of Energy under the Grant No. DE-AC36-08GO28308. NR 28 TC 28 Z9 28 U1 1 U2 48 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD NOV 1 PY 2012 VL 112 IS 9 AR 093717 DI 10.1063/1.4759322 PG 6 WC Physics, Applied SC Physics GA 049FS UT WOS:000311968400064 ER PT J AU Ma, C Qin, YB Yang, HX Tian, HF Li, JQ Sardar, K Walton, RI Su, D Wu, LJ Zhu, YM AF Ma, Chao Qin, Yuanbin Yang, Huaixin Tian, Huanfang Li, Jianqi Sardar, Kripasindhu Walton, Richard I. Su, Dong Wu, Lijun Zhu, Yimei TI Microstructure and oxidation states in multiferroic Lu-2(Fe,Mn)(3)O-7 SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID FERROELECTRICITY; LUFE2O4 AB Microstructural features and oxidation states in multiferroic Lu2Fe2.1Mn0.9O7 have been investigated by neutron diffraction, transmission electron microscopy (TEM), and x-ray absorption near edge spectroscopy. Our experimental results demonstrate the disordered distribution of Mn atoms in the FeO double (W) layers, indicating that structural modulations originate from the charge disproportionation, which is evidenced by the mixed-valence states of Fe ions. TEM measurements clearly reveal Mn doping induced chemical inhomogeneity and local distortions which are associated with the charge disproportionation in the W layers. In addition, the polarization is discussed in association with the lattice distortions and charge disproportionation. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4764309] C1 [Ma, Chao; Qin, Yuanbin; Yang, Huaixin; Tian, Huanfang; Li, Jianqi] Chinese Acad Sci, Inst Phys, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China. [Sardar, Kripasindhu; Walton, Richard I.] Univ Warwick, Dept Chem, Coventry CV4 7AL, W Midlands, England. [Su, Dong; Wu, Lijun; Zhu, Yimei] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Li, JQ (reprint author), Chinese Acad Sci, Inst Phys, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China. EM ljq@aphy.iphy.ac.cn RI Su, Dong/A-8233-2013; Ma, Chao/J-4569-2015 OI Su, Dong/0000-0002-1921-6683; FU National Basic Research Program of China 973 Program [2011CBA00101, 2011CB921703, 2010CB923002, 2012CB821404]; National Natural Science Foundation of China [90922001, 10904166, 11274368, 51272277, 11074292, 11004229, 11190022]; Chinese Academy of Sciences; U.S. Department of Energy, Office of Basic Energy Science, Division of Materials Science and Engineering [DE-AC02-98CH10886]; University of Warwick FX We would like to thank Y. Li for her help during TEM sample preparation. Work at Institute of Physics, CAS, was supported by National Basic Research Program of China 973 Program (Grant Nos. 2011CBA00101, 2011CB921703, 2010CB923002, 2012CB821404), the National Natural Science Foundation of China (Grant Nos. 90922001, 10904166, 11274368, 51272277, 11074292, 11004229, 11190022), and Chinese Academy of Sciences. Work at Brookhaven was supported by the U.S. Department of Energy, Office of Basic Energy Science, Division of Materials Science and Engineering, under Contract No. DE-AC02-98CH10886. We are grateful to the University of Warwick for the award of a Strategic Partnership Fund grant. NR 25 TC 1 Z9 1 U1 3 U2 36 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 J9 J APPL PHYS JI J. Appl. Phys. PD NOV 1 PY 2012 VL 112 IS 9 AR 094105 DI 10.1063/1.4764309 PG 5 WC Physics, Applied SC Physics GA 049FS UT WOS:000311968400089 ER PT J AU Motyka, MA Gauntt, BD Horn, MW Dickey, EC Podraza, NJ AF Motyka, M. A. Gauntt, B. D. Horn, M. W. Dickey, E. C. Podraza, N. J. TI Microstructural evolution of thin film vanadium oxide prepared by pulsed-direct current magnetron sputtering SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID TIME SPECTROSCOPIC ELLIPSOMETRY; TEMPERATURE-DEPENDENCE; DIELECTRIC FUNCTION; CRITICAL-POINTS; STOICHIOMETRY; TRANSITION; DIOXIDE; SILICON; GE; SI AB Vanadium oxide (VOx) thin films have been deposited by pulsed-DC magnetron sputtering using a metallic vanadium target in a reactive argon and oxygen environment. While the process parameters (power, total pressure, oxygen-to-argon ratio) remained constant, the deposition time was varied to produce films between 75 +/- 6 and 2901 +/- 30 angstrom thick, which were then optically and electrically characterized. The complex dielectric function spectra (epsilon = epsilon(1) + i epsilon(2)) of the films from 0.75 to 5.15 eV were extracted by ex situ, multiple-angle spectroscopic ellipsometry (SE) measurements for the series of varied thickness VOx samples. Significant changes in epsilon and resistivity occur as a function of thickness, indicating the correlations exist between the electrical and the optical properties over this spectral range. In addition, in situ measurements via real time SE (RTSE) were made on the film grown to the largest thickness to track optical property and structural variations during growth. RTSE was also used to characterize changes in the film occurring after growth was completed, namely during post sputtering in the presence of argon and oxygen while the sample is shielded, and atmospheric exposure. RTSE indicates that the exposure of the film to the argon and oxygen environment, regardless of the shutter isolating the target, causes up to 200 angstrom of the top surface of the deposited film to become more electrically resistive as evidenced by variations in epsilon. Exposure of the VOx thin film to atmospheric conditions introduces a similar change in epsilon, but this change occurs throughout the bulk of the film. A combination of these observations with RTSE results indicates that thinner, less ordered VOx films are more susceptible to drastic changes due to atmospheric exposure and that microstructural variations in this material ultimately control its environmental stability. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4759255] C1 [Motyka, M. A.; Horn, M. W.] Penn State Univ, Dept Engn Sci & Mech, University Pk, PA 16802 USA. [Gauntt, B. D.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Dickey, E. C.] N Carolina State Univ, Dept Mat Sci & Engn, Raleigh, NC 27606 USA. [Podraza, N. J.] Univ Toledo, Dept Phys & Astron, Toledo, OH 43606 USA. RP Motyka, MA (reprint author), Penn State Univ, Dept Engn Sci & Mech, 227 Hammond Bldg, University Pk, PA 16802 USA. EM mamotyka00@gmail.com RI Dickey, Elizabeth/A-3368-2011 OI Dickey, Elizabeth/0000-0003-4005-7872 FU U.S. Army Research Office [W911NF-0-2-0026]; U.S. Army Research Laboratory [W911NF-0-2-0026] FX The U.S. Army Research Office and U.S. Army Research Laboratory sponsored this research under Cooperative Agreement No. W911NF-0-2-0026. NR 19 TC 3 Z9 3 U1 1 U2 43 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 J9 J APPL PHYS JI J. Appl. Phys. PD NOV 1 PY 2012 VL 112 IS 9 AR 093504 DI 10.1063/1.4759255 PG 6 WC Physics, Applied SC Physics GA 049FS UT WOS:000311968400025 ER PT J AU Solis, KJ Martin, JE AF Solis, Kyle J. Martin, James E. TI Controlling the column spacing in isothermal magnetic advection to enable tunable heat and mass transfer SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID FERROFLUIDS; COMPOSITES; FIELD AB Isothermal magnetic advection (IMA) is a recently discovered method of inducing highly organized, non-contact flow lattices in suspensions of magnetic particles, using only uniform ac magnetic fields of modest strength. The initiation of these vigorous flows requires neither a thermal gradient nor a gravitational field, and so can be used to transfer heat and mass in circumstances where natural convection does not occur. These advection lattices are comprised of a square lattice of antiparallel flow columns. If the column spacing is sufficiently large compared to the column length and the flow rate within the columns is sufficiently large, then one would expect efficient transfer of both heat and mass. Otherwise, the flow lattice could act as a countercurrent heat exchanger and only mass will be efficiently transferred. Although this latter case might be useful for feeding a reaction front without extracting heat, it is likely that most interest will be focused on using IMA for heat transfer. In this paper, we explore the various experimental parameters of IMA to determine which of these can be used to control the column spacing. These parameters include the field frequency, strength, and phase relation between the two field components, the liquid viscosity, and particle volume fraction. We find that the column spacing can easily be tuned over a wide range to enable the careful control of heat and mass transfer. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4764308] C1 [Solis, Kyle J.; Martin, James E.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Solis, KJ (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; Division of Materials Science, Office of Basic Energy Sciences, U.S. Department of Energy (DOE) FX Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. This work was supported by the Division of Materials Science, Office of Basic Energy Sciences, U.S. Department of Energy (DOE). We thank Vladimir Raksha, Paul Coombs, Tom Markantes, Bill Kittler, and Kees-Jan Delst at JDSU for supplying the magnetic platelets. NR 11 TC 1 Z9 1 U1 0 U2 4 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0021-8979 J9 J APPL PHYS JI J. Appl. Phys. PD NOV 1 PY 2012 VL 112 IS 9 AR 094912 DI 10.1063/1.4764308 PG 7 WC Physics, Applied SC Physics GA 049FS UT WOS:000311968400144 ER PT J AU Chen, M Wang, XR Qi, HR Shankar, M AF Chen, Ming Wang, Xiaorui Qi, Hairong Shankar, Mallikarjun TI Adaptive response time control for metadata matching in information dissemination systems SO JOURNAL OF SYSTEMS ARCHITECTURE LA English DT Article DE Information dissemination; Response time; Feedback control; Metadata matching; Adaptive control; Real-time systems ID DATABASES; ALGORITHMS AB Information dissemination is of increasing importance to our society. Existing work mainly focuses on delivering information from sources to sinks in a timely manner based on established subscriptions, with the assumption that those subscriptions are persistent. However, the bottleneck of many information dissemination systems is actually the matching process to continuously reevaluate such subscriptions between numerous sources and numerous sinks, in response to dynamically varying information attributes at runtime. In this paper, we propose an adaptive control architecture to meet the response time constraints on metadata matching in an example information dissemination system. Our adaptive controller features a rigorous design based on well-established control theory for guaranteed control accuracy and system stability. Furthermore, our controller can adapt to changes in the system model without reconfiguration and profiling. Empirical results on a physical testbed demonstrate that our controller has more accurate control and improved system quality of service than both an open-loop solution and a typical heuristic solution. (C) 2012 Elsevier B.V. All rights reserved. C1 [Wang, Xiaorui] Ohio State Univ, Columbus, OH 43210 USA. [Chen, Ming; Qi, Hairong] Univ Tennessee, Knoxville, TN 37996 USA. [Shankar, Mallikarjun] Oak Ridge Natl Lab, Oak Ridge, TN 37830 USA. RP Wang, XR (reprint author), Ohio State Univ, Columbus, OH 43210 USA. EM xwang@ece.osu.edu RI Shankar, Mallikarjun/N-4400-2015; Wang, Xiaorui/L-2774-2016 OI Shankar, Mallikarjun/0000-0001-5289-7460; Wang, Xiaorui/0000-0001-9633-1418 FU NSF [CNS-0845390, CNS- 0720663]; Department of Homeland Security; Laboratory Directed Research and Development Program of Oak Ridge National Laboratory [DE-AC05-00OR22725] FX This research is supported in part by NSF under Grants CNS-0845390 and CNS- 0720663 and by a subcontract from the Department of Homeland Security-sponsored Southeast Region Research Initiative (SERRI) at the National Nuclear Security Administration's Y-12 National Security Complex, and by the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory under Contract No. DE-AC05-00OR22725. We would also like to thank Dieter Gawlick at Oracle Corporation for his help with the INFOD system. NR 36 TC 0 Z9 0 U1 0 U2 4 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 1383-7621 J9 J SYST ARCHITECT JI J. Syst. Architect. PD NOV PY 2012 VL 58 IS 10 BP 412 EP 425 DI 10.1016/j.sysarc.2012.08.003 PG 14 WC Computer Science, Hardware & Architecture; Computer Science, Software Engineering SC Computer Science GA 052CK UT WOS:000312175100003 ER PT J AU Bulanov, SV Esirkepov, TZ Kando, M Koga, JK Pirozhkov, AS Nakamura, T Bulanov, SS Schroeder, CB Esarey, E Califano, F Pegoraro, F AF Bulanov, Sergei V. Esirkepov, Timur Zh. Kando, Masaki Koga, James K. Pirozhkov, Alexander S. Nakamura, Tatsufumi Bulanov, Stepan S. Schroeder, Carl B. Esarey, Eric Califano, Francesco Pegoraro, Francesco TI On the breaking of a plasma wave in a thermal plasma. I. The structure of the density singularity SO PHYSICS OF PLASMAS LA English DT Article ID WAKE-FIELD ACCELERATION; ELECTRON-ACCELERATORS; UNDERDENSE PLASMA; LASER-PULSES; OSCILLATIONS; IONIZATION; TRANSITION; INJECTION; EQUATION; REGIME AB The structure of the singularity that is formed in a relativistically large amplitude plasma wave close to the wave breaking limit is found by using a simple waterbag electron distribution function. The electron density distribution in the breaking wave has a typical "peakon" form. The maximum value of the electric field in a thermal breaking plasma is obtained and compared to the cold plasma limit. The results of computer simulations for different initial electron distribution functions are in agreement with the theoretical conclusions. The after-wavebreak regime is then examined, and a semi-analytical model of the density evolution is constructed. Finally the results of two dimensional particle in cell simulations for different initial electron distribution functions are compared, and the role of thermal effects in enhancing particle injection is noted. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4764052] C1 [Bulanov, Sergei V.; Esirkepov, Timur Zh.; Kando, Masaki; Koga, James K.; Pirozhkov, Alexander S.; Nakamura, Tatsufumi] Japan Atom Energy Agcy, QuBS, Kizugawa, Kyoto 6190215, Japan. [Schroeder, Carl B.; Esarey, Eric] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Califano, Francesco; Pegoraro, Francesco] Univ Pisa, Dept Phys, I-56127 Pisa, Italy. [Bulanov, Sergei V.] RAS, AM Prokhorov Inst Gen Phys, Moscow 117901, Russia. [Bulanov, Stepan S.] Inst Theoret & Expt Phys, Moscow 117218, Russia. RP Bulanov, SV (reprint author), Japan Atom Energy Agcy, QuBS, 1-8-7 Umemidai, Kizugawa, Kyoto 6190215, Japan. RI Bulanov, Sergei/A-1721-2013; OI Schroeder, Carl/0000-0002-9610-0166 FU MEXT of Japan; MEXT [23740413, 21740302]; NSF [PHY-0935197]; Office of Science of the US DOE [DE-AC02-05CH11231] FX We thank A. G. Zhidkov and M. Lobet for discussions. We acknowledge support of this work from the MEXT of Japan, Grant-in-Aid for Scientific Research, 23740413, and Grant-in-Aid for Young Scientists 21740302 from MEXT. We appreciate support from the NSF under Grant No. PHY-0935197 and the Office of Science of the US DOE under Contract No. DE-AC02-05CH11231. NR 72 TC 10 Z9 10 U1 1 U2 22 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 1070-664X J9 PHYS PLASMAS JI Phys. Plasmas PD NOV PY 2012 VL 19 IS 11 AR 113102 DI 10.1063/1.4764052 PG 14 WC Physics, Fluids & Plasmas SC Physics GA 050DS UT WOS:000312033700044 ER PT J AU Bulanov, SV Esirkepov, TZ Kando, M Koga, JK Pirozhkov, AS Nakamura, T Bulanov, SS Schroeder, CB Esarey, E Califano, F Pegoraro, F AF Bulanov, Sergei V. Esirkepov, Timur Zh. Kando, Masaki Koga, James K. Pirozhkov, Alexander S. Nakamura, Tatsufumi Bulanov, Stepan S. Schroeder, Carl B. Esarey, Eric Califano, Francesco Pegoraro, Francesco TI On the breaking of a plasma wave in a thermal plasma. II. Electromagnetic wave interaction with the breaking plasma wave SO PHYSICS OF PLASMAS LA English DT Article ID NONLINEAR PHOTON ACCELERATOR; ULTRASHORT LASER-PULSES; RELATIVISTIC PLASMA; DISPERSION; WAKE AB In thermal plasma, the structure of the density singularity formed in a relativistically large amplitude plasma wave close to the wavebreaking limit leads to a refraction coefficient with discontinuous spatial derivatives. This results in a non-exponentially small above-barrier reflection of an electromagnetic wave interacting with the nonlinear plasma wave. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4764056] C1 [Bulanov, Sergei V.; Esirkepov, Timur Zh.; Kando, Masaki; Koga, James K.; Pirozhkov, Alexander S.; Nakamura, Tatsufumi] Japan Atom Energy Agcy, QuBS, Kizugawa, Kyoto 6190215, Japan. [Schroeder, Carl B.; Esarey, Eric] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Califano, Francesco; Pegoraro, Francesco] Univ Pisa, Dept Phys, I-56127 Pisa, Italy. [Bulanov, Sergei V.] RAS, AM Prokhorov Inst Gen Phys, Moscow 117901, Russia. [Bulanov, Stepan S.] Inst Theoret & Expt Phys, Moscow 117218, Russia. RP Bulanov, SV (reprint author), Japan Atom Energy Agcy, QuBS, 1-8-7 Umemidai, Kizugawa, Kyoto 6190215, Japan. RI Bulanov, Sergei/A-1721-2013; OI Schroeder, Carl/0000-0002-9610-0166 FU MEXT of Japan; MEXT [23740413, 21740302]; NSF [PHY-0935197]; Office of Science of the US DOE [DE-AC02-05CH11231] FX We thank M. Lobet for discussions. We acknowledge the support from the MEXT of Japan, Grant-in-Aid for Scientific Research, 23740413, and Grant-in-Aid for Young Scientists 21740302 from MEXT. We appreciate support from the NSF under Grant No. PHY-0935197 and the Office of Science of the US DOE under Contract No. DE-AC02-05CH11231. NR 53 TC 6 Z9 6 U1 1 U2 12 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 1070-664X J9 PHYS PLASMAS JI Phys. Plasmas PD NOV PY 2012 VL 19 IS 11 AR 113103 DI 10.1063/1.4764056 PG 7 WC Physics, Fluids & Plasmas SC Physics GA 050DS UT WOS:000312033700045 ER PT J AU Chen, LJ Daughton, W Bhattacharjee, A Torbert, RB Roytershteyn, V Bessho, N AF Chen, Li-Jen Daughton, William Bhattacharjee, Amitava Torbert, Roy B. Roytershteyn, Vadim Bessho, Naoki TI In-plane electric fields in magnetic islands during collisionless magnetic reconnection SO PHYSICS OF PLASMAS LA English DT Article ID PLASMA SHEET; ACCELERATION; REGION AB Magnetic islands are a common feature in both the onset and nonlinear evolution of magnetic reconnection. In collisionless regimes, the onset typically occurs within ion-scale current layers leading to the formation of magnetic islands when multiple X lines are involved. The nonlinear evolution of reconnection often gives rise to extended electron current layers (ECL) which are also unstable to formation of magnetic islands. Here, we show that the excess negative charge and strong out-of-plane electron velocity in the ECL are passed on to the islands generated therein, and that the corresponding observable distinguishing the islands generated in the ECL is the strongly enhanced in-plane electric fields near the island core. The islands formed in ion-scale current layers do not have these properties of the ECL-generated islands. The above result provides a way to assess the occurrence and importance of extended ECLs that are unstable to island formation in space and laboratory plasmas. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4767645] C1 [Chen, Li-Jen; Bhattacharjee, Amitava; Torbert, Roy B.; Bessho, Naoki] Univ New Hampshire, Ctr Space Sci, Durham, NH 03824 USA. [Daughton, William] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Roytershteyn, Vadim] Univ Calif San Diego, La Jolla, CA 92093 USA. RP Chen, LJ (reprint author), Univ New Hampshire, Ctr Space Sci, Durham, NH 03824 USA. RI Daughton, William/L-9661-2013; NASA MMS, Science Team/J-5393-2013; OI NASA MMS, Science Team/0000-0002-9504-5214; Roytershteyn, Vadim/0000-0003-1745-7587 FU DOE [DE-FG02-07ER54941]; NSF [PHY-0903923, ATM-090315, AGS-0962698]; NASA [NNH11AQ451]; NASAs Heliophysics Theory Program; DOE through the LANL/LDRD program FX The research at UNH was supported in part by DOE DE-FG02-07ER54941, NSF PHY-0903923, NSF ATM-090315, NSF AGS-0962698, and NASA NNH11AQ451. Contributions from W. D. and V. R. were supported by NASAs Heliophysics Theory Program and by the DOE through the LANL/LDRD program. We are grateful for computer time provided by the ASC program on the Roadrunner machine, LANL institutional computing resources, and an allocation on Kraken supported by the NSF at the National Institute for Computational Sciences. NR 26 TC 12 Z9 12 U1 1 U2 17 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 1070-664X J9 PHYS PLASMAS JI Phys. Plasmas PD NOV PY 2012 VL 19 IS 11 AR 112902 DI 10.1063/1.4767645 PG 7 WC Physics, Fluids & Plasmas SC Physics GA 050DS UT WOS:000312033700041 ER PT J AU Ellis, IN Strozzi, DJ Winjum, BJ Tsung, FS Grismayer, T Mori, WB Fahlen, JE Williams, EA AF Ellis, I. N. Strozzi, D. J. Winjum, B. J. Tsung, F. S. Grismayer, T. Mori, W. B. Fahlen, J. E. Williams, E. A. TI Convective Raman amplification of light pulses causing kinetic inflation in inertial fusion plasmas SO PHYSICS OF PLASMAS LA English DT Article ID PARTICLE-IN-CELL; STIMULATED RAMAN; ELECTROMAGNETIC-WAVES; SCATTERING; BACKSCATTER; DRIVEN; SIMULATION; BRILLOUIN; MODEL AB We perform 1D particle-in-cell (PIC) simulations using OSIRIS, which model a short-duration (similar to 500 omega(-1)(0) FWHM) scattered light seed pulse in the presence of a constant counter-propagating pump laser with an intensity far below the absolute instability threshold. The seed undergoes linear convective Raman amplification and dominates over fluctuations due to particle discreteness. Our simulation results are in good agreement with results from a coupled-mode solver when we take into account special relativity and the use of finite size PIC simulation particles. We present linear gain spectra including both effects. Extending the PIC simulations past when the seed exits the simulation domain reveals bursts of large-amplitude scattering in many cases, which does not occur in simulations without the seed pulse. These bursts can have amplitudes several times greater than the amplified seed pulse, and we demonstrate that this large-amplitude scattering is the result of kinetic inflation by examining trapped particle orbits. This large-amplitude scattering is caused by the seed modifying the distribution function earlier in the simulation. We perform some simulations with longer duration seeds, which lead to parts of the seeds undergoing kinetic inflation and reaching amplitudes several times more than the steady-state linear theory results. Simulations with continuous seeds demonstrate that the onset of inflation depends on seed wavelength and incident intensity, and we observe oscillations in the reflectivity at a frequency equal to the difference between the seed frequency and the frequency at which the inflationary stimulated Raman scattering grows. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4762853] C1 [Ellis, I. N.; Strozzi, D. J.; Williams, E. A.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Ellis, I. N.; Winjum, B. J.; Tsung, F. S.; Grismayer, T.; Mori, W. B.; Fahlen, J. E.] Univ Calif Los Angeles, Los Angeles, CA 90095 USA. [Grismayer, T.] Inst Super Tecn, Grp Lasers & Plasmas, P-1049001 Lisbon, Portugal. RP Ellis, IN (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM ellis@physics.ucla.edu RI Grismayer, Thomas/J-4850-2013; OI Grismayer, Thomas/0000-0002-0045-389X; Strozzi, David/0000-0001-8814-3791 FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; University of California, Los Angeles [FG52-09NA29552, DE-NA0001833]; Laboratory Directed Research and Development Program at LLNL [08-ERD-017]; Lawrence Scholar Program at LLNL FX This work performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344 and by the University of California, Los Angeles under Grants FG52-09NA29552 and DE-NA0001833. This work was funded in part by the Laboratory Directed Research and Development Program at LLNL under project tracking code 08-ERD-017. Work by I. N. Ellis was supported in part by the Lawrence Scholar Program at LLNL. NR 48 TC 6 Z9 6 U1 0 U2 25 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 1070-664X J9 PHYS PLASMAS JI Phys. Plasmas PD NOV PY 2012 VL 19 IS 11 AR 112704 DI 10.1063/1.4762853 PG 15 WC Physics, Fluids & Plasmas SC Physics GA 050DS UT WOS:000312033700035 ER PT J AU Gueroult, R Fisch, NJ AF Gueroult, Renaud Fisch, Nathaniel J. TI Particle deconfinement in a bent magnetic mirror SO PHYSICS OF PLASMAS LA English DT Article ID TANDEM MIRROR; MASS FILTER; PLASMA AB Coils misalignment in a magnetic mirror can produce additional particle transport. The magnetic field non axi-symmetry is responsible for radial and longitudinal drifts in a way much similar to the neo-classical transport in a tandem mirror cell distorted by end plugs. Accordingly, a regime exhibiting large radial displacements-similar to the resonant regime in tandem mirrors-can be obtained by confining ions azimuthally, for example by means of a properly tuned radial electric field. Because of the mass dependence of the magnetic field non-homogeneity drift velocities, the azimuthal trapping is mass specific, allowing, in principle, the filtering of a specific species based on its mass. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4765692] C1 [Gueroult, Renaud; Fisch, Nathaniel J.] Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. RP Gueroult, R (reprint author), Princeton Univ, Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA. FU US DOE [DE-FG02-06ER54851, DE-AC02-09CH11466] FX This work was supported by US DOE under Contract Nos. DE-FG02-06ER54851 and DE-AC02-09CH11466. NR 23 TC 0 Z9 0 U1 0 U2 6 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 1070-664X J9 PHYS PLASMAS JI Phys. Plasmas PD NOV PY 2012 VL 19 IS 11 AR 112105 DI 10.1063/1.4765692 PG 6 WC Physics, Fluids & Plasmas SC Physics GA 050DS UT WOS:000312033700007 ER PT J AU Hudson, SR Dewar, RL Dennis, G Hole, MJ McGann, M von Nessi, G Lazerson, S AF Hudson, S. R. Dewar, R. L. Dennis, G. Hole, M. J. McGann, M. von Nessi, G. Lazerson, S. TI Computation of multi-region relaxed magnetohydrodynamic equilibria SO PHYSICS OF PLASMAS LA English DT Article ID PLASMA-VACUUM SYSTEMS; SURFACE CURRENT EQUILIBRIA; FORCE-FREE FIELDS; MAGNETIC-FIELDS; HAMILTONIAN-SYSTEMS; MHD EQUILIBRIA; SPECTRAL CODE; STABILITY; PRESSURE; ISLANDS AB We describe the construction of stepped-pressure equilibria as extrema of a multi-region, relaxed magnetohydrodynamic (MHD) energy functional that combines elements of ideal MHD and Taylor relaxation, and which we call MRXMHD. The model is compatible with Hamiltonian chaos theory and allows the three-dimensional MHD equilibrium problem to be formulated in a well-posed manner suitable for computation. The energy-functional is discretized using a mixed finite-element, Fourier representation for the magnetic vector potential and the equilibrium geometry; and numerical solutions are constructed using the stepped-pressure equilibrium code, SPEC. Convergence studies with respect to radial and Fourier resolution are presented. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4765691] C1 [Hudson, S. R.; Lazerson, S.] Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. [Dewar, R. L.; Dennis, G.; Hole, M. J.; McGann, M.; von Nessi, G.] Australian Natl Univ, Plasma Res Lab, Res Sch Phys & Engn, Canberra, ACT 0200, Australia. RP Hudson, SR (reprint author), Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA. EM shudson@pppl.gov; robert.dewar@anu.edu.au; graham.dennis@anu.edu.au; matthew.hole@anu.edu.au; mathew.mcgann@anu.edu.au; greg.vonnessi@anu.edu.au; slazerso@pppl.gov RI Hudson, Stuart/H-7186-2013; Dewar, Robert/B-1300-2008; Lazerson, Samuel/E-4816-2014 OI Hudson, Stuart/0000-0003-1530-2733; Dewar, Robert/0000-0002-9518-7087; Lazerson, Samuel/0000-0001-8002-0121 FU Australian Research Council [DP0452728, FT0991899, DP110102881]; U.S. Department of Energy FX We dedicate this article to Paul Garabedian, whom we consider to be a pioneer in the field of 3D MHD calculations and also endorsed and employed weak solutions.106 We are also indebted to Steve Hirshman, who has provided VMEC. One of us (S. R. H.) acknowledges stimulating discussions with Neil Pomphrey, with Don Monticello regarding the construction of straight-field-line coordinates, and with Allen Boozer regarding the choice of gauge107 for the vector potential, and R. L. D. acknowledges discussion with Robert MacKay. The authors gratefully acknowledge support of the U.S. Department of Energy and the Australian Research Council, through Grants DP0452728, FT0991899, and DP110102881. NR 106 TC 28 Z9 28 U1 1 U2 16 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD NOV PY 2012 VL 19 IS 11 AR 112502 DI 10.1063/1.4765691 PG 18 WC Physics, Fluids & Plasmas SC Physics GA 050DS UT WOS:000312033700027 ER PT J AU Ng, J Egedal, J Le, A Daughton, W AF Ng, J. Egedal, J. Le, A. Daughton, W. TI Phase space structure of the electron diffusion region in reconnection with weak guide fields SO PHYSICS OF PLASMAS LA English DT Article ID COLLISIONLESS DRIVEN RECONNECTION; MAGNETIC RECONNECTION AB Kinetic simulations of magnetic reconnection provide detailed information about the electric and magnetic structure throughout the simulation domain, as well as high resolution profiles of the essential fluid parameters including the electron and ion densities, flows, and pressure tensors. However, the electron distribution function, f(v), within the electron diffusion region becomes highly structured in the three dimensional velocity space and is not well resolved by the data available from the particle-in-cell (PIC) simulations. Here, we reconstruct the electron distribution function within the diffusion region at enhanced resolution. This is achieved by tracing electron orbits in the fields taken from PIC simulations back to the inflow region where an analytic form of the magnetized electron distribution is known. For antiparallel reconnection, the analysis reveals the highly structured nature of f(v), with striations corresponding to the number of times electrons have been reflected within the reconnection current layer, and exposes the origin of gradients in the electron pressure tensor important for momentum balance. The structure of the reconnection region is strongly tied to the pressure anisotropy that develops in the electrons upstream of the reconnection region. The addition of a guide field changes the nature of the electron distributions, and the differences are accounted for by studying the motion of single particles in the field geometry. Finally, the geometry of small guide field reconnection is shown to be highly sensitive to the ion/electron mass ratio applied in the simulation. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4766895] C1 [Ng, J.; Egedal, J.; Le, A.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Ng, J.; Egedal, J.; Le, A.] MIT, Plasma Sci & Fus Ctr, Cambridge, MA 02139 USA. [Daughton, W.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Ng, J (reprint author), MIT, Dept Phys, Cambridge, MA 02139 USA. EM jegedal@psfc.mit.edu RI Daughton, William/L-9661-2013 FU NASA (National Aeronautics and Space Administration) at MIT [NNX10AL11G]; National Science Foundation (NSF) at MIT [0844620]; NASA Heliophysics Theory Program at LANL FX We gratefully acknowledge support from NASA (National Aeronautics and Space Administration) through Grant NNX10AL11G, and National Science Foundation (NSF) CAREER Grant 0844620 (both at MIT) and by the NASA Heliophysics Theory Program at LANL. Simulations were carried out using LANL institutional computing resources and the Pleiades computer at NASA. NR 28 TC 19 Z9 19 U1 0 U2 6 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 1070-664X J9 PHYS PLASMAS JI Phys. Plasmas PD NOV PY 2012 VL 19 IS 11 AR 112108 DI 10.1063/1.4766895 PG 12 WC Physics, Fluids & Plasmas SC Physics GA 050DS UT WOS:000312033700010 ER PT J AU Stacey, WM Boedo, JA Evans, TE Grierson, BA Groebner, RJ AF Stacey, W. M. Boedo, J. A. Evans, T. E. Grierson, B. A. Groebner, R. J. TI Intrinsic rotation produced by ion orbit loss and X-loss SO PHYSICS OF PLASMAS LA English DT Article ID SCRAPE-OFF-LAYER; ALCATOR C-MOD; TOKAMAK PLASMA; TOROIDAL ROTATION; TRANSPORT; EDGE; SEPARATRIX; FLOWS; FIELD AB A practical calculation model for the intrinsic rotation imparted to the edge plasma by the directionally preferential loss of ions on orbits that cross the last closed flux surface is presented and applied to calculate intrinsic rotation in several DIII-D [J. Luxon, Nucl. Fusion 42, 614 ( 2002)] discharges. The intrinsic rotation produced by ion loss is found to be sensitive to the edge temperature and radial electric field profiles, which has implications for driving intrinsic rotation in future large tokamaks. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4768424] C1 [Stacey, W. M.] Georgia Inst Technol, Atlanta, GA 30332 USA. [Boedo, J. A.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Evans, T. E.; Groebner, R. J.] Gen Atom Co, San Diego, CA 92186 USA. [Grierson, B. A.] Princeton Plasma Phys Lab, Princeton, NJ 08453 USA. RP Stacey, WM (reprint author), Georgia Inst Technol, Atlanta, GA 30332 USA. FU U. S. Department of Energy [DE-FG02-99ER54538, DE-AC03-99ER54463]; Georgia Tech Research Corporation; General Atomics FX The first author is grateful to John deGrassie for a couple of useful discussions on the subject and to General Atomics for their hospitality during the course of some of the work reported in this paper. The contributions of other members of the DIII-D Team are gratefully acknowledged. This work was supported by the U. S. Department of Energy through Grant No. DE-FG02-99ER54538 with the Georgia Tech Research Corporation and through Contract No. DE-AC03-99ER54463 with General Atomics. NR 37 TC 16 Z9 16 U1 0 U2 5 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 1070-664X J9 PHYS PLASMAS JI Phys. Plasmas PD NOV PY 2012 VL 19 IS 11 AR 112503 DI 10.1063/1.4768424 PG 8 WC Physics, Fluids & Plasmas SC Physics GA 050DS UT WOS:000312033700028 ER PT J AU Strozzi, DJ Williams, EA Rose, HA Hinkel, DE Langdon, AB Banks, JW AF Strozzi, D. J. Williams, E. A. Rose, H. A. Hinkel, D. E. Langdon, A. B. Banks, J. W. TI Threshold for electron trapping nonlinearity in Langmuir waves SO PHYSICS OF PLASMAS LA English DT Article ID NATIONAL-IGNITION-FACILITY; PLASMA-WAVES; PARAMETRIC-INSTABILITIES; STIMULATED RAMAN; FREQUENCY-SHIFT; LASER-BEAMS; DRIVEN; LIGHT; OSCILLATIONS; SCATTERING AB We assess when electron trapping nonlinearity is expected to be important in Langmuir waves. The basic criterion is that the inverse of the detrapping rate nu(d) of electrons in the trapping region of velocity space must exceed the bounce period of deeply trapped electrons, tau(B) (n(e)/delta n)(1/2)2 pi/omega(pe). A unitless figure of merit, the "bounce number" N-B 1/nu(d)tau(B), encapsulates this condition and defines a trapping threshold amplitude for which N-B = 1. The detrapping rate is found for convective loss (transverse and longitudinal) out of a spatially finite Langmuir wave. Simulations of driven waves with a finite transverse profile, using the 2D-2V Vlasov code LOKI, show trapping nonlinearity increases continuously with N-B for transverse loss, and is significant for N-B approximate to 1. The detrapping rate due to Coulomb collisions (both electron-electron and electron-ion) is also found, with pitch-angle scattering and parallel drag and diffusion treated in a unified manner. A simple way to combine convective and collisional detrapping is given. Application to underdense plasma conditions in inertial confinement fusion targets is presented. The results show that convective transverse loss is usually the most potent detrapping process in a single f/8 laser speckle. For typical plasma and laser conditions on the inner laser cones of the National Ignition Facility, local reflectivities similar to 3% are estimated to produce significant trapping effects. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4767644] C1 [Strozzi, D. J.; Williams, E. A.; Hinkel, D. E.; Langdon, A. B.; Banks, J. W.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Rose, H. A.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Strozzi, DJ (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. EM strozzi2@llnl.gov RI Banks, Jeffrey/A-9718-2012; OI Strozzi, David/0000-0001-8814-3791 FU US Department of Energy under LDRD Tracking [DE-AC52-07NA27344, 12-ERD-061] FX We gratefully recognize J. A. F. Hittinger and R. L. Berger for helpful discussions and support. Work at LLNL was supported by US Department of Energy Contract No. DE-AC52-07NA27344 and partly under LDRD Tracking No. 12-ERD-061. NR 56 TC 12 Z9 12 U1 0 U2 14 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 1070-664X J9 PHYS PLASMAS JI Phys. Plasmas PD NOV PY 2012 VL 19 IS 11 AR 112306 DI 10.1063/1.4767644 PG 14 WC Physics, Fluids & Plasmas SC Physics GA 050DS UT WOS:000312033700024 ER PT J AU Terry, MR Perkins, LJ Sepke, SM AF Terry, Matthew R. Perkins, L. John Sepke, Scott M. TI Design of a deuterium and tritium-ablator shock ignition target for the National Ignition Facility SO PHYSICS OF PLASMAS LA English DT Article ID POLAR-DIRECT-DRIVE; SIMULATIONS; PERFORMANCE; INSTABILITY; RADIOGRAPHY; INTENSITY; SYSTEM; OMEGA AB Shock ignition presents a viable path to ignition and high gain on the National Ignition Facility (NIF). In this paper, we describe the development of the 1D design of 0.5MJ class, all-deuterium and tritium (fuel and ablator) shock ignition target that should be reasonably robust to Rayleigh-Taylor fluid instabilities, mistiming, and hot electron preheat. The target assumes "day one" NIF hardware and produces a yield of 31MJ with reasonable allowances for laser backscatter, absorption efficiency, and polar drive power variation. The energetics of polar drive laser absorption require a beam configuration with half of the NIF quads dedicated to launching the ignitor shock, while the remaining quads drive the target compression. Hydrodynamic scaling of the target suggests that gains of 75 and yields 70MJ may be possible. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4765354] C1 [Terry, Matthew R.; Perkins, L. John; Sepke, Scott M.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Terry, MR (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. EM terry10@llnl.gov FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 62 TC 8 Z9 8 U1 0 U2 18 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 1070-664X J9 PHYS PLASMAS JI Phys. Plasmas PD NOV PY 2012 VL 19 IS 11 AR 112705 DI 10.1063/1.4765354 PG 13 WC Physics, Fluids & Plasmas SC Physics GA 050DS UT WOS:000312033700036 ER PT J AU Maezawa, Y Umeda, T Aoki, S Ejiri, S Hatsuda, T Kanaya, K Ohno, H AF Maezawa, Yu Umeda, Takashi Aoki, Sinya Ejiri, Shinji Hatsuda, Tetsuo Kanaya, Kazuyuki Ohno, Hiroshi CA WHOT-QCD Collaboration TI Application of Fixed Scale Approach to Static Quark Free Energies in Quenched and 2+1 Flavor Lattice QCD with Improved Wilson Quark Action SO PROGRESS OF THEORETICAL PHYSICS LA English DT Article ID FINITE-TEMPERATURE AB The free energies of static quarks and the Debye screening masses in the quark gluon plasma are studied using Polyakov-line correlation functions in lattice QCD adopting the fixed-scale approach in which temperature is varied without changing the spatial volume and the renormalization factors. We calculate static-quark free energies in various color channels in the high temperature phase up to about 3.5 times the (pseudo-)critical temperature, performing lattice simulations both in quenched and 2+1 flavor QCD. For the quenched simulations, we adopt the plaquette gauge action on anisotropic 20(3) x N-t lattices with N-t = 8-26 at the renormalized anisotropy a(s)/a(t) similar or equal to 4. For 2 + 1 flavor QCD, we adopt the renormalization-group improved Iwasaki gluon action and the non-perturbatively O(alpha)-improved Wilson quark action on isotropic 32(3) x N-t lattices with N-t = 4-12 at m(PS)/m(V) = 0.63 (0.74) for the light (strange) flavors. We find that the color-singlet free energies at high temperatures converge to the zero-temperature static-quark potential evaluated from the Wilson-loop at short distances. This is in accordance with the theoretical expectation that the short distance physics is insensitive to the temperature. At long distances, the free energies approach twice the single-quark free energies, implying that the interaction between static quarks is fully screened. We find that the static-quark free energies for various color channels turn out to be well described by the screened Coulomb form, and the color-channel dependence of the inter-quark interaction can be described by the kinetic Casimir factor inspired from the lowest order perturbation theory. We also discuss comparison with a prediction of the thermal perturbation theory and flavor dependence of the screening masses. C1 [Maezawa, Yu] RIKEN, Nishina Ctr, Phys Math Lab, Wako, Saitama 3510198, Japan. [Umeda, Takashi] Hiroshima Univ, Grad Sch Educ, Higashihiroshima 7398524, Japan. [Aoki, Sinya; Kanaya, Kazuyuki] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki 3058571, Japan. [Aoki, Sinya] Univ Tsukuba, Ctr Computat Sci, Tsukuba, Ibaraki 3058577, Japan. [Ejiri, Shinji] Niigata Univ, Grad Sch Sci & Technol, Niigata 9502181, Japan. [Hatsuda, Tetsuo] RIKEN, Nishina Ctr, Theoret Res Div, Wako, Saitama 3510198, Japan. [Hatsuda, Tetsuo] Univ Tokyo, IPMU, Kashiwa, Chiba 2778583, Japan. [Ohno, Hiroshi] Univ Tsukuba, Grad Sch Pure & Appl Sci, Tsukuba, Ibaraki 3058571, Japan. RP Maezawa, Y (reprint author), Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. RI Hatsuda, Tetsuo/C-2901-2013 FU Grants-in-Aid of the Japanese Ministry of Education, Culture, Sports, Science and Technology [22740168, 21340049, 20340047, 23540295]; Grant-in-Aid for Scientific Research on Innovative Areas [2004: 20105001, 20105003, 2310576]; Large Scale Simulation Program of High Energy Accelerator Research Organization (KEK) [09/10-25, 10-09]; RIKEN Integrated Cluster of Cluster (RICC) facility FX We thank the members of the CP-PACS and JLQCD Collaborations for providing us with their high-statistics 2+1 flavor QCD configurations at T = 0, and also the authors of Ref. 30) for providing us with the results of their static-quark potential fit. YM would like to thank Koichi Yazaki for useful discussions. HO is supported by the Japan Society for the Promotion of Science for Young Scientists. This work is in part supported by Grants-in-Aid of the Japanese Ministry of Education, Culture, Sports, Science and Technology (Nos. 22740168, 21340049, 20340047, 23540295). SA, SE and TH are supported in part by the Grant-in-Aid for Scientific Research on Innovative Areas (No. 2004: 20105001, 20105003, 2310576). This work is in part supported also by the Large Scale Simulation Program of High Energy Accelerator Research Organization (KEK) Nos. 09/10-25 and 10-09, and the RIKEN Integrated Cluster of Cluster (RICC) facility. NR 36 TC 9 Z9 9 U1 0 U2 0 PU PROGRESS THEORETICAL PHYSICS PUBLICATION OFFICE PI KYOTO PA C/O KYOTO UNIV, YUKAWA HALL, KYOTO, 606-8502, JAPAN SN 0033-068X J9 PROG THEOR PHYS JI Prog. Theor. Phys. PD NOV PY 2012 VL 128 IS 5 BP 955 EP 970 PG 16 WC Physics, Multidisciplinary SC Physics GA 051JB UT WOS:000312121400009 ER PT J AU Ren, PY Chun, JH Thomas, DG Schnieders, MJ Marucho, M Zhang, JJ Baker, NA AF Ren, Pengyu Chun, Jaehun Thomas, Dennis G. Schnieders, Michael J. Marucho, Marcelo Zhang, Jiajing Baker, Nathan A. TI Biomolecular electrostatics and solvation: a computational perspective SO QUARTERLY REVIEWS OF BIOPHYSICS LA English DT Review ID POISSON-BOLTZMANN EQUATION; MOLECULAR-DYNAMICS SIMULATIONS; INTERACTION-SITE-MODEL; POLARIZABLE FORCE-FIELD; GENERALIZED-BORN MODEL; HYDRATION FREE-ENERGY; DENSITY-FUNCTIONAL THEORY; IMPLICIT SOLVENT MODELS; DISTRIBUTED MULTIPOLE ANALYSIS; CENTERED DIELECTRIC FUNCTIONS AB An understanding of molecular interactions is essential for insight into biological systems at the molecular scale. Among the various components of molecular interactions, electrostatics are of special importance because of their long-range nature and their influence on polar or charged molecules, including water, aqueous ions, proteins, nucleic acids, carbohydrates, and membrane lipids. In particular, robust models of electrostatic interactions are essential for understanding the solvation properties of biomolecules and the effects of solvation upon biomolecular folding, binding, enzyme catalysis, and dynamics. Electrostatics, therefore, are of central importance to understanding biomolecular structure and modeling interactions within and among biological molecules. This review discusses the solvation of biomolecules with a computational biophysics view toward describing the phenomenon. While our main focus lies on the computational aspect of the models, we provide an overview of the basic elements of biomolecular solvation (e.g. solvent structure, polarization, ion binding, and non-polar behavior) in order to provide a background to understand the different types of solvation models. C1 [Chun, Jaehun; Thomas, Dennis G.; Baker, Nathan A.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Ren, Pengyu; Schnieders, Michael J.; Zhang, Jiajing] Univ Texas Austin, Dept Biomed Engn, Austin, TX 78712 USA. [Marucho, Marcelo] Univ Texas San Antonio, Dept Phys & Astron, San Antonio, TX 78249 USA. RP Baker, NA (reprint author), Pacific NW Natl Lab, POB 999,MSID K7-29, Richland, WA 99352 USA. EM nathan.baker@pnnl.gov RI Baker, Nathan/A-8605-2010 OI Baker, Nathan/0000-0002-5892-6506 FU NIH [R01 GM069702, P41 RR0860516, R01 GM076121-04S1, R01 GM090208-01] FX The authors would like to thank Cornelia Brim for her help in preparing the manuscript, Greg Schenter for his review and insightful comments, and Andy McCammon for his patience with this very overdue review. This work was supported by NIH grants R01 GM069702, P41 RR0860516, R01 GM076121-04S1, and R01 GM090208-01. NR 745 TC 50 Z9 51 U1 16 U2 269 PU CAMBRIDGE UNIV PRESS PI NEW YORK PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA SN 0033-5835 J9 Q REV BIOPHYS JI Q. Rev. Biophys. PD NOV PY 2012 VL 45 IS 4 BP 427 EP 491 DI 10.1017/S003358351200011X PG 65 WC Biophysics SC Biophysics GA 050NA UT WOS:000312058800002 PM 23217364 ER PT J AU Chapman, JL Morris, MD Anderson-Cook, CM AF Chapman, Jessica L. Morris, Max D. Anderson-Cook, Christine M. TI Computationally Efficient Comparison of Experimental Designs for System Reliability Studies With Binomial Data SO TECHNOMETRICS LA English DT Article DE Complex systems; Markov chain Monte Carlo; Resource allocation ID BAYESIAN-ESTIMATION; SERIES; SUBSYSTEMS; COMPONENTS AB A common practical problem in experimental design is that of quantitatively determining how to best use a fixed amount of resources to supplement an existing analysis with additional data. We address this problem in the context of the second stage in Bayesian system reliability studies; these second-stage data are aimed at obtaining a more precise estimate of the system's reliability. The current strategy for comparing potential experimental designs is computationally intensive and time-consuming. We present new, more computationally efficient methodology that can be used to quickly assess the anticipated improvements for candidate allocations, and demonstrate its effectiveness with a missile system application. While we find that there are some situations in which our methodology may provide a more optimistic estimate of the expected improvement to be gained from a candidate experiment than the current approach, the results of the two methods tend to closely match when the rankings of candidate experiments are considered. Our implementation of the algorithm (in C), along with a brief description and an example input set, is available online as supplementary materials. C1 [Chapman, Jessica L.] St Lawrence Univ, Dept Math Comp Sci & Stat, Canton, NY 13617 USA. [Morris, Max D.] Iowa State Univ, Dept Stat, Ames, IA 50011 USA. [Anderson-Cook, Christine M.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Chapman, JL (reprint author), St Lawrence Univ, Dept Math Comp Sci & Stat, Canton, NY 13617 USA. EM jchapman@stlawu.edu; mmorris@iastate.edu; c-and-cook@lanl.gov FU NSF [DMS 0502347 EMSW21-RTG, 0959713] FX This work was funded in part by an NSF grant DMS 0502347 EMSW21-RTG awarded to Iowa State University and an NSF award 0959713 awarded to St. Lawrence University. The authors thank the editor, associate editor, and two anonymous referees whose constructive feedback on earlier versions greatly improved the final article. NR 20 TC 2 Z9 2 U1 2 U2 4 PU AMER STATISTICAL ASSOC PI ALEXANDRIA PA 732 N WASHINGTON ST, ALEXANDRIA, VA 22314-1943 USA SN 0040-1706 J9 TECHNOMETRICS JI Technometrics PD NOV PY 2012 VL 54 IS 4 BP 410 EP 424 DI 10.1080/00401706.2012.694784 PG 15 WC Statistics & Probability SC Mathematics GA 050LE UT WOS:000312054000009 ER PT J AU Hochanadel, PW Field, RD Lewis, GK AF Hochanadel, P. W. Field, R. D. Lewis, G. K. TI MICROSTRUCTURE AND PROPERTIES OF LASER DEPOSITED AND WROUGHT ALLOY K-500 (UNS N05500) SO WELDING IN THE WORLD LA English DT Article DE Deposition; Dissimilar; Metals; Laser; Metallurgy; Nickel Alloys ID PHASE-CHANGE; MONEL K-500; KINETICS; PRECIPITATION AB Feasibility tests were performed by manufacturing transition joints between Nickel-200 (Ni-200) and Alloy K-500 (K-500) with direct laser deposition. Both sharp and functionally graded interfaces were manufactured with no apparent issues. In addition, Alloy K-500 specimens were manufactured with direct laser deposition to analyze the isothermal hardening response of Alloy K-500. The laser deposited and wrought materials were precipitation hardened at three different temperatures (600 degrees C, 650 degrees C, and 700 degrees C) and various times. A relationship between the hardness and the volume fraction of Ni-3(Ti,Al) was developed, and the subsequent analysis showed that the corresponding Johnson-Mehl-Avrami time constants (or n-values) ranged from 1.1 to 1.3 at an aging temperature 600 degrees C, and decreased to values ranging from 0.6 to 0.66 at an aging temperature of 700 degrees C. For site saturation and spherical precipitates, the expected n-value is 1.5. This analysis showed that the mechanism for precipitation changed as a function of temperature. The results of the analysis at higher temperatures were rationalized by the possibility of the decay of quenched-in vacancies, precipitation along the grain boundaries, and precipitation along the dislocations. It was, however, difficult to confirm these possibilities with transmission electron microscopy (TEM), since imaging the precipites is difficult at very early aging times. Finally, it was determined that the heat treatment schedule of laser welded or laser clad Alloy K-500 should be similar to that of wrought Alloy K-500. C1 [Hochanadel, P. W.; Field, R. D.; Lewis, G. K.] Los Alamos Natl Lab, Los Alamos, NM USA. RP Hochanadel, PW (reprint author), Los Alamos Natl Lab, Los Alamos, NM USA. FU National Nuclear Security Administration of the U.S. Department of Energy [DE-AC52-06NA25396] FX This work was performed at Los Alamos National Laboratory, an affirmative action/equal opportunity employer, operated by the Los Alamos National Security, LLC for the National Nuclear Security Administration of the U.S. Department of Energy under contract DE-AC52-06NA25396. NR 15 TC 1 Z9 1 U1 3 U2 16 PU INT INST WELDING PI 95942 ROISSY CH DE GAULLE CEDEX PA BP 51362, 95942 ROISSY CH DE GAULLE CEDEX, 00000, FRANCE SN 0043-2288 J9 WELD WORLD JI Weld. World PD NOV-DEC PY 2012 VL 56 IS 11-12 BP 51 EP 58 PG 8 WC Metallurgy & Metallurgical Engineering SC Metallurgy & Metallurgical Engineering GA 038SX UT WOS:000311195500006 ER PT J AU Madan, D Wang, ZQ Chen, A Juang, RC Keist, J Wright, PK Evans, JW AF Madan, Deepa Wang, Zuoqian Chen, Alic Juang, Rei-cheng Keist, Jay Wright, Paul K. Evans, Jim W. TI Enhanced Performance of Dispenser Printed MA n-type Bi2Te3 Composite Thermoelectric Generators SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE dispenser-printer; mechanical alloyed Bi2Te3; composite thermoelectric materials; energy harvesting; thermoelectric generators; Se additive ID ELECTRICAL-PROPERTIES; OPTIMIZATION; DEFECTS AB This work presents performance advancements of dispenser printed composite thermoelectric materials and devices. Dispenser printed thick films allow for low-cost and scalable manufacturing of microscale energy harvesting devices. A maximum ZT value of 0.31 has been achieved for mechanically alloyed (MA) n-type Bi2Te3-epoxy composite films with 1 wt % Se cured at 350 degrees C. The enhancement of ZT is a result of increase in the electrical conductivity through the addition of Se, which ultimately lowers the sintering temperature (350 degrees C). A 62 single-leg thermoelectric generator (TEG) prototype with 5 mm x700 mu m x 120 mu m printed element dimensions was fabricated on a custom designed polyimide substrate with thick metal contacts. The prototype device produced a power output of 25 mu W at 0.23 mA current and 109 mV voltage for a temperature difference of 20 degrees C, which is sufficient for low power generation for autonomous microsystem applications. C1 [Madan, Deepa; Wang, Zuoqian; Chen, Alic; Wright, Paul K.] Univ Calif Berkeley, Dept Mech Engn, Berkeley, CA 94720 USA. [Keist, Jay; Evans, Jim W.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Juang, Rei-cheng] Ind Technol Res Inst, Green Energy & Environm Res Lab, Hsinchu 310, Taiwan. [Keist, Jay] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94550 USA. RP Madan, D (reprint author), Univ Calif Berkeley, Dept Mech Engn, Berkeley, CA 94720 USA. EM deepam@berkeley.edu RI Wang, Zuoqian/I-9562-2014 OI Wang, Zuoqian/0000-0002-6587-1187 FU California Energy Commission [500-01-43] FX The authors thank the California Energy Commission for supporting this research under contract 500-01-43. We also thank Michael Nill, Jonathan Brown, Brian Mahlstedt, Kevin Huang, and Rich Winslow for their contributions. NR 39 TC 18 Z9 18 U1 10 U2 72 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD NOV PY 2012 VL 4 IS 11 BP 6117 EP 6124 DI 10.1021/am301759a PG 8 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA 043DA UT WOS:000311521900053 PM 23130550 ER PT J AU Van Gough, D Bunker, BC Roberts, ME Huber, DL Zarick, HF Austin, MJ Wheeler, JS Moore, D Spoerke, ED AF Van Gough, Dara Bunker, Bruce C. Roberts, Mark E. Huber, Dale L. Zarick, Holly F. Austin, Mariah J. Wheeler, Jill S. Moore, Diana Spoerke, Erik D. TI Thermally Programmable pH Buffers SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE PNIPAM; buffer; programmable; thermally responsive; pH; copolymer ID CHEMICAL BATH DEPOSITION; N-ISOPROPYLACRYLAMIDE; MICROGELS; ACID AB Many reactions in both chemistry and biology rely on the ability to precisely control and fix the solution concentrations of either protons or hydroxide ions. In this report, we describe the behavior of thermally programmable pH buffer systems based on the copolymerization of varying amounts of acrylic acid (AA) groups into N-isopropylacrylamide polymers. Because the copolymers undergo phase transitions upon heating and cooling, the local environment around the AA groups can be reversibly switched between hydrophobic and hydrophilic states affecting the ionization behavior of the acids. Results show that moderate temperature variations can be used to change the solution pH by two units. However, results also indicate that the nature of the transition and its impact on the pH values are highly dependent on the AA content and the degree of neutralization. C1 [Van Gough, Dara; Bunker, Bruce C.; Huber, Dale L.; Zarick, Holly F.] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA. RP Van Gough, D (reprint author), Sandia Natl Labs, Ctr Integrated Nanotechnol, POB 5800, Albuquerque, NM 87185 USA. EM dgough@sandia.gov RI Huber, Dale/A-6006-2008; Roberts, Mark/H-9865-2016 OI Huber, Dale/0000-0001-6872-8469; Roberts, Mark/0000-0001-5971-6650 FU Laboratory Directed Research and Development; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This research was supported by Laboratory Directed Research and Development funding at Sandia National Laboratories. This work was performed, in part, at the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences, user facility. Sandia National Laboratories is a multi-program laboratory operated by Sandia Corp., a wholly owned subsidiary of Lockheed Martin Co. for the U.S. Department of Energy's National Nuclear Security Administration, under Contract DE-AC04-94AL85000. The authors also acknowledge Dr. Andrew D. Price for helpful discussion. NR 18 TC 4 Z9 4 U1 1 U2 13 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD NOV PY 2012 VL 4 IS 11 BP 6247 EP 6251 DI 10.1021/am301836p PG 5 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA 043DA UT WOS:000311521900070 PM 23130670 ER PT J AU Yeo, SJ Shin, SH Nam, KT Yoo, PJ AF Yeo, Seon Ju Shin, Seong-Ho Nam, Ki Tae Yoo, Pil J. TI Multidimensional Assembly of S-Layer Proteins on Mobility-Controlled Polyelectrolyte Multilayers SO ACS MACRO LETTERS LA English DT Article ID ATOMIC-FORCE MICROSCOPY; SILICON SUPPORTS; GROWTH; RECRYSTALLIZATION; POLYCATIONS; DIFFUSION; SURFACES; LATTICES; EXCHANGE AB Polyelectrolyte multilayers have been vastly utilized as an assembling platform for various biomaterials because of their soft and charged surface characteristics, analogous to biomembrane systems. In particular, polyelectrolyte chains with high self-diffusivity can effectively transfer the surface mobility to the assembling biomolecular species, facilitating the ordered self-assembly. Herein, highly diffusional cationic polyelectrolyte chains of linear polyethylenimine are employed to induce direct binding with negatively charged bacterial surface layer proteins, which eventually lead to largescale two-dimensional crystals. Notably, at the elevated incubation temperature, a transitory intermediate of one-dimensional chain structure is observed. We reveal that this one-dimensional intermediate is a stable precursor toward two-dimensional crystal arrays. C1 [Nam, Ki Tae] Seoul Natl Univ, Dept Mat Sci & Engn, Seoul 151744, South Korea. [Yeo, Seon Ju; Yoo, Pil J.] Sungkyunkwan Univ, Sch Chem Engn, Suwon 440746, South Korea. [Yoo, Pil J.] Sungkyunkwan Univ, SKKU Adv Inst Nanotechnol SAINT, Suwon 440746, South Korea. [Shin, Seong-Ho] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry & Mat Sci Div, Berkeley, CA 94720 USA. RP Nam, KT (reprint author), Seoul Natl Univ, Dept Mat Sci & Engn, Seoul 151744, South Korea. EM nkitae@snu.ac.kr; pjyoo@skku.edu RI Yoo, Pil J./A-1069-2012 OI Yoo, Pil J./0000-0002-5499-6566 FU Basic Science Research Program [2010-0009877, 2010-0029409, 2012-0004117]; National Research Foundation of Korea (NRF) [NRF-C1AAA001-2010-0028962]; Korea Government (MEST); Global Frontier R&D Program on Center for Multiscale Energy System [2011-0031574] FX This work was supported by Basic Science Research Program grants (2010-0009877, 2010-0029409, 2012-0004117) and research grant (NRF-C1AAA001-2010-0028962) through the National Research Foundation of Korea (NRF) funded by the Korea Government (MEST). K.T.N. appreciates support by the Global Frontier R&D Program on Center for Multiscale Energy System (2011-0031574). NR 26 TC 1 Z9 1 U1 2 U2 20 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2161-1653 J9 ACS MACRO LETT JI ACS Macro Lett. PD NOV PY 2012 VL 1 IS 11 BP 1254 EP 1257 DI 10.1021/mz3004538 PG 4 WC Polymer Science SC Polymer Science GA 043DD UT WOS:000311522200007 ER PT J AU Lu, CH Remington, BA Maddox, BR Kad, B Park, HS Prisbrey, ST Meyers, MA AF Lu, C. H. Remington, B. A. Maddox, B. R. Kad, B. Park, H. S. Prisbrey, S. T. Meyers, M. A. TI Laser compression of monocrystalline tantalum SO ACTA MATERIALIA LA English DT Article DE Dislocation; Laser treatment; Tantalum; Twinning; Shock compression ID COPPER-ALUMINUM ALLOYS; SHOCK COMPRESSION; PLASTIC ANISOTROPY; SINGLE-CRYSTALS; FLOW-STRESS; DEFORMATION; TRANSITION; PRESSURE; TUNGSTEN; METALS AB Monocrystalline tantalum with orientations [1 0 0] and [1 1 1] was subjected to laser-driven compression at energies of 350-684 J, generating shock amplitudes varying from 10 to 110 GPa. A stagnating reservoir driven by a laser beam with a spot radius of 800 mu m created a crater of significant depth (similar to 80 to similar to 200 mu m) on the drive side of the Ta sample. The defects generated by the laser pulse were characterized by transmission and scanning electron microscopy, and are composed of dislocations at low pressures, and mechanical twins and a displacive phase transformation at higher pressures. The defect substructure is a function of distance from the energy deposition surface and correlates directly with the pressure. Directly under the bottom of the crater is an isentropic layer, approximately 40 mu m thick, which shows few deformation markings. Lattice rotation was observed immediately beneath this layer. Further below this regime, a high density of twins and dislocations was observed. As the shock amplitude decayed to below similar to 40 GPa, the incidence of twinning decreased dramatically, suggesting a critical threshold pressure. The twinning planes were primarily {1 1 2}, although some {1 2 3} twins were also observed. Body-centered cubic to hexagonal close-packed pressure induced-transformation was observed at high pressures (similar to 68 GPa). The experimentally measured dislocation densities and threshold stress for twinning are compared with predictions using analyses based on the constitutive response, and the similarities and differences are discussed in terms of the mechanisms of defect generation. (C) 2012 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Lu, C. H.; Kad, B.; Meyers, M. A.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Remington, B. A.; Maddox, B. R.; Park, H. S.; Prisbrey, S. T.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Meyers, MA (reprint author), Univ Calif San Diego, La Jolla, CA 92093 USA. EM mameyers@ucsd.edu RI Meyers, Marc/A-2970-2016 OI Meyers, Marc/0000-0003-1698-5396 FU UC Research Laboratories [09-LR-06-118456-MEYM]; National Laser Users Facility (NLUF) [PE-FG52-09NA-29043]; Division of Scientific User Facilities, US Department of Energy; NI grants FX This research is funded by a UC Research Laboratories Grant (09-LR-06-118456-MEYM) and a National Laser Users Facility (NLUF) Grant (PE-FG52-09NA-29043). We thank T. Remington for yield stress measurement, C.T. Wei for help with the manuscript preparation, Rain Luo for profilometry measurement, Dr. Fabienne Gregori for her hospitality at the Universite Paris Nord and for transmission electron microscopy, and Dr. Y. Tang for overall assistance. Electron microscopy was conducted at the SHaRE User Facility, which is sponsored at Oak Ridge National Laboratory by the Division of Scientific User Facilities, US Department of Energy. We acknowledge the use of the UCSD Cryo-Electron Microscopy Facility, which is supported by NI grants to Dr. Timothy S. Baker and a gift from the Agouron Institute to UCSD. NR 62 TC 30 Z9 30 U1 5 U2 49 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 J9 ACTA MATER JI Acta Mater. PD NOV PY 2012 VL 60 IS 19 BP 6601 EP 6620 DI 10.1016/j.actamat.2012.08.026 PG 20 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA 038QE UT WOS:000311188400016 ER PT J AU Cakmak, E Choo, H An, K Ren, Y AF Cakmak, Ercan Choo, Hahn An, Ke Ren, Yang TI A synchrotron X-ray diffraction study on the phase transformation kinetics and texture evolution of a TRIP steel subjected to torsional loading SO ACTA MATERIALIA LA English DT Article DE Synchrotron diffraction Torsional deformation; Martensitic phase transformation; Transformation kinetics; Texture evolution ID INDUCED MARTENSITIC-TRANSFORMATION; AUSTENITIC STAINLESS-STEEL; FREE END TORSION; PLASTIC-DEFORMATION; NEUTRON-DIFFRACTION; VARIANT SELECTION; STRAIN-RATE; MULTIPHASE STEELS; RATE SENSITIVITY; AXIAL STRESSES AB The martensitic phase transformation kinetics and the relation with texture evolution in the constituent phases were studied for a transformation-induced plasticity (TRIP) steel under a torsional loading condition at ambient temperature. Synchrotron X-ray diffraction was used to measure the evolution of phase fractions and texture in terms of pole figures and orientation distribution functions as a function of the applied shear strain. The effects of deformation texture development in the parent austenite phase on the observed phase transformation kinetics are discussed in terms of preferred transformation mechanisms. The texture evolution in the product martensite phase is also discussed in terms of possible texture inheritance from the parent austenite phase and its own deformation texture. Published by Elsevier Ltd. on behalf of Acta Materialia Inc. C1 [Cakmak, Ercan; Choo, Hahn] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [An, Ke] Oak Ridge Natl Lab, Spallat Neutron Source, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. [Ren, Yang] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. RP Choo, H (reprint author), Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. EM hchoo@utk.edu RI Choo, Hahn/A-5494-2009; An, Ke/G-5226-2011; Cakmak, Ercan/J-8605-2014 OI Choo, Hahn/0000-0002-8006-8907; An, Ke/0000-0002-6093-429X; FU NSF [DMR.0421219]; Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy [DE-AC02-06C1-111357] FX This research was supported in part by the NSF Major Research Instrumentation program under contract DMR.0421219. Use of the Advanced Photon Source was supported by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy, under contract no. DE-AC02-06C1-111357. The work at Oak Ridge National Laboratory was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. The authors would like to acknowledge Mr. Harley Skorpenske (Oak Ridge National Laboratory) for his help using the load frame and Mr. Douglas Fielden (University of Tennessee) for machining the specimens. NR 51 TC 11 Z9 11 U1 1 U2 49 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 J9 ACTA MATER JI Acta Mater. PD NOV PY 2012 VL 60 IS 19 BP 6703 EP 6713 DI 10.1016/j.actamat.2012.08.040 PG 11 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA 038QE UT WOS:000311188400025 ER PT J AU Wan, HB Shen, Y Wang, J Shen, ZQ Jin, XJ AF Wan, Haibo Shen, Yao Wang, Jian Shen, Zhiqiang Jin, Xuejun TI A predictive model for microstructure evolution in metallic multilayers with immiscible constituents SO ACTA MATERIALIA LA English DT Article DE Metallic multilayers; Zig-zag microstructure; Triple junction; Pinch-off; High-temperature stability ID GRAIN-BOUNDARY MOTION; FINITE-ELEMENT-METHOD; SIMULATING INTERFACE MOTION; TRIPLE JUNCTION MOTION; THIN-FILMS; SURFACE-DIFFUSION; THERMAL-STABILITY; CAPILLARY; INTERDIFFUSION; INSTABILITIES AB Focussing on the thermal stability of layered structures, we developed a predictive model to study the microstructure evolution of metallic multilayers with different morphologies including aligned and classical staggered grain geometries. We found that the zig-zag microstructure experimentally observed in multilayers forms when grains in each upper layer have a relative shift less than half the in-plane grain size to the lower layer. During this formation process, the non-equilibrium triple junctions move, driven by the imbalance of tensions of interphase and grain boundaries, corresponding to an extension to classical grooving theory. Numerical simulations show that a finite mobility of the triple junction can effectively impede the development of grooves, suggesting that the classical t(1/4) dependence of groove depth with the assumption of an infinite triple junction mobility might be questionable at low temperatures to predict the time to pinch-off. Further, a map for the stability of layered structure in Cu/Nb system is developed in terms of the aspect ratio of grain dimensions and the ratio of the distance between two nearest triple junctions to the in-plane grain size. A criterion for this stability is also proposed for multilayers with similar grain boundary energies based on simplified geometrical consideration. Both the map and the simple criterion are in good agreement with the experiments for Cu/Nb multilayers. (C) 2012 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Wan, Haibo; Shen, Yao; Shen, Zhiqiang; Jin, Xuejun] Shanghai Jiao Tong Univ, State Key Lab Met Matrix Composites, Sch Mat Sci & Engn, Shanghai 200240, Peoples R China. [Wan, Haibo] Shanghai Power Equipment Res Inst, Shanghai 200240, Peoples R China. [Wang, Jian] Los Alamos Natl Lab, Mat Sci & Technol Div, Los Alamos, NM 87545 USA. RP Shen, Y (reprint author), Shanghai Jiao Tong Univ, State Key Lab Met Matrix Composites, Sch Mat Sci & Engn, Shanghai 200240, Peoples R China. EM yaoshen@sjtu.edu.cn RI Wang, Jian/F-2669-2012 OI Wang, Jian/0000-0001-5130-300X FU National Science Foundation of China (NSFC) [50971090]; State Key Development Program for Basic Research of China (973 Programs) [2012CB619600]; NSFC [50601018, 50890174]; US Department of Energy, Office of Science, Office of Basic Energy Sciences; Los Alamos National Laboratory Directed Research and Development (LDRD) [ER20110573] FX The research was supported by National Science Foundation of China (NSFC) under Project No. 50971090, and by State Key Development Program for Basic Research of China (973 Programs) (Grant No. 2012CB619600). Y.S. is grateful for the financial support of the NSFC under Project Nos. 50601018 and 50890174. J.W. also acknowledges support provided by the US Department of Energy, Office of Science, Office of Basic Energy Sciences and a Los Alamos National Laboratory Directed Research and Development (LDRD) Project ER20110573. NR 47 TC 10 Z9 10 U1 0 U2 34 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 J9 ACTA MATER JI Acta Mater. PD NOV PY 2012 VL 60 IS 19 BP 6869 EP 6881 DI 10.1016/j.actamat.2012.08.062 PG 13 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA 038QE UT WOS:000311188400042 ER PT J AU Appel, AA Chou, CY Greisler, HP Larson, JC Vasireddi, S Zhong, Z Anastasio, MA Brey, EM AF Appel, Alyssa A. Chou, Cheng-Ying Greisler, Howard P. Larson, Jeffery C. Vasireddi, Sunil Zhong, Zhong Anastasio, Mark A. Brey, Eric M. TI Analyzer-based phase-contrast x-ray imaging of carotid plaque microstructure SO AMERICAN JOURNAL OF SURGERY LA English DT Article DE Phase contrast X-ray imaging; Carotid stenosis; Cardiovascular imaging; Computerized tomography ID ARTICULAR-CARTILAGE; IMPLEMENTATION; RADIOGRAPHY AB BACKGROUND: Plaque vulnerability depends, in part, on composition. Imaging techniques are needed that can aid the prediction of plaque stability. High-contrast images of soft-tissue structure have been obtained with x-ray phase-contrast (PC) imaging. This research investigates multiple image radiography (MIR), an x-ray PC imaging technique, for evaluation of human carotid artery plaques. METHODS: Carotid plaques were imaged with ultrasound and subsequently excised and formalin fixed. MIR imaging was performed. By using synchrotron radiation, conventional radiographs were acquired for comparison. Image texture measures were computed for soft-tissue regions of the plaques. RESULTS: Ultrasound evaluation identified plaques as homogeneous without calcifications. MIR images revealed complex heterogeneous structure with multiple microcalcifications consistent with histology, and possessed more image texture in specific regions than conventional radiographs (P < .05). MIR refraction images allowed imaging of the geometric structure of tissue interfaces within the plaques, while scatter images contained more texture in soft-tissue regions than absorption or refraction images. CONCLUSIONS: X-ray PC imaging better depicts plaque soft-tissue heterogeneity than ultrasound or conventional radiographs. MIR imaging technique should be investigated further as a viable imaging technique to identify high-risk plaques. (C) 2012 Elsevier Inc. All rights reserved. C1 [Appel, Alyssa A.; Greisler, Howard P.; Larson, Jeffery C.; Brey, Eric M.] Hines VA Hosp, Dept Res, Hines, IL 60616 USA. [Appel, Alyssa A.; Larson, Jeffery C.; Vasireddi, Sunil; Brey, Eric M.] IIT, Dept Biomed Engn, Pritzker Inst Biomed Sci & Engn, Chicago, IL 60616 USA. [Chou, Cheng-Ying] Natl Taiwan Univ, Dept Bioind Mechatron Engn, Taipei 10764, Taiwan. [Greisler, Howard P.] Loyola Med Sch, Dept Surg, Maywood, IL USA. [Greisler, Howard P.] Loyola Med Sch, Dept Cell Biol Neurobiol & Anat, Maywood, IL USA. [Zhong, Zhong] Brookhaven Natl Lab, Natl Synchrotron Light Source, Upton, NY 11973 USA. [Anastasio, Mark A.] Washington Univ, Dept Biomed Engn, St Louis, MO USA. RP Brey, EM (reprint author), Hines VA Hosp, Dept Res, Hines, IL 60616 USA. EM brey@iit.edu OI CHOU, CHENG-YING/0000-0002-5737-6960 FU National Institutes of Health [EB009715]; National Science Foundation [CBET 1135068]; Veterans Administration FX This research was supported by National Institutes of Health grant EB009715, National Science Foundation grant CBET 1135068, and the Veterans Administration The authors thank Dr. Jovan Brankov for his advice on CT imaging. NR 17 TC 3 Z9 3 U1 1 U2 5 PU EXCERPTA MEDICA INC-ELSEVIER SCIENCE INC PI BRIDGEWATER PA 685 ROUTE 202-206 STE 3, BRIDGEWATER, NJ 08807 USA SN 0002-9610 J9 AM J SURG JI Am. J. Surg. PD NOV PY 2012 VL 204 IS 5 BP 631 EP 636 DI 10.1016/j.amjsurg.2012.07.021 PG 6 WC Surgery SC Surgery GA 045YZ UT WOS:000311734000020 PM 23140828 ER PT J AU Moeller, SJ Hajcak, G Parvaz, MA Dunning, JP Volkow, ND Goldstein, RZ AF Moeller, Scott J. Hajcak, Greg Parvaz, Muhammad A. Dunning, Jonathan P. Volkow, Nora D. Goldstein, Rita Z. TI Psychophysiological prediction of choice: relevance to insight and drug addiction SO BRAIN LA English DT Article DE cocaine addiction; insight; choice behaviour; event-related potentials; late positive potential; unconscious motivation ID CURRENT COCAINE USERS; ATTENTIONAL BIAS; MOTIVATED ATTENTION; EMOTION REGULATION; HEROIN DEPENDENCE; NEURAL RESPONSES; MONETARY REWARD; CUES; BRAIN; ASSOCIATIONS AB An important goal of addiction research and treatment is to predict behavioural responses to drug-related stimuli. This goal is especially important for patients with impaired insight, which can interfere with therapeutic interventions and potentially invalidate self-report questionnaires. This research tested (i) whether event-related potentials, specifically the late positive potential, predict choice to view cocaine images in cocaine addiction; and (ii) whether such behaviour prediction differs by insight (operationalized in this study as self-awareness of image choice). Fifty-nine cocaine abusers and 32 healthy controls provided data for the following laboratory components that were completed in a fixed-sequence (to establish prediction): (i) event-related potential recordings while passively viewing pleasant, unpleasant, neutral and cocaine images, during which early (400-1000 ms) and late (1000-2000 ms) window late positive potentials were collected; (ii) self-reported arousal ratings for each picture; and (iii) two previously validated tasks: one to assess choice for viewing these same images, and the other to group cocaine abusers by insight. Results showed that pleasant-related late positive potentials and arousal ratings predicted pleasant choice (the choice to view pleasant pictures) in all subjects, validating the method. In the cocaine abusers, the predictive ability of the late positive potentials and arousal ratings depended on insight. Cocaine-related late positive potentials better predicted cocaine image choice in cocaine abusers with impaired insight. Another emotion-relevant event-related potential component (the early posterior negativity) did not show these results, indicating specificity of the late positive potential. In contrast, arousal ratings better predicted respective cocaine image choice (and actual cocaine use severity) in cocaine abusers with intact insight. Taken together, the late positive potential could serve as a biomarker to help predict drug-related choice-and possibly associated behaviours (e.g. drug seeking in natural settings, relapse after treatment)-when insight (and self-report) is compromised. C1 [Moeller, Scott J.; Parvaz, Muhammad A.; Goldstein, Rita Z.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Hajcak, Greg] SUNY Stony Brook, Dept Psychol, Stony Brook, NY 11794 USA. [Dunning, Jonathan P.] Nevada State Coll, Dept Social Sci, Henderson, NV 89002 USA. [Volkow, Nora D.] NIDA, Bethesda, MD 20892 USA. [Volkow, Nora D.] NIAAA, Bethesda, MD 20892 USA. RP Goldstein, RZ (reprint author), Brookhaven Natl Lab, 30 Bell Ave,Bldg 490, Upton, NY 11973 USA. EM rgoldstein@bnl.gov RI Moeller, Scott/L-5549-2016; OI Moeller, Scott/0000-0002-4449-0844; Parvaz, Muhammad/0000-0002-2671-2327 FU U.S. Department of Energy [DE-AC02-98CHI-886]; National Institute on Drug Abuse [1R01DA023579, 1F32DA030017-01] FX The authors gratefully acknowledge the contributions of Thomas Maloney, Patricia A. Woicik, Nelly Alia-Klein, Frank Telang, Gene-Jack Wang and Nicasia Beebe-Wang. This article has been authored by Brookhaven Science Associates, LLC under Contract No. DE-AC02-98CHI-886 with the U.S. Department of Energy. The United States Government retains, and the publisher, by accepting the article for publication, acknowledges, a world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for the United States Government purposes.; This study was supported by grants from the National Institute on Drug Abuse (to R.Z.G.: 1R01DA023579; to S.J.M.: 1F32DA030017-01). NR 59 TC 18 Z9 18 U1 3 U2 23 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0006-8950 J9 BRAIN JI Brain PD NOV PY 2012 VL 135 BP 3481 EP 3494 DI 10.1093/brain/aws252 PN 11 PG 14 WC Clinical Neurology; Neurosciences SC Neurosciences & Neurology GA 044SV UT WOS:000311644800031 PM 23148349 ER PT J AU Young, RM Neumark, DM AF Young, Ryan M. Neumark, Daniel M. TI Dynamics of Solvated Electrons in Clusters SO CHEMICAL REVIEWS LA English DT Review ID PUMP-PROBE SPECTROSCOPY; INITIO MOLECULAR-DYNAMICS; RESOLVED PHOTOELECTRON-SPECTROSCOPY; TRANSIENT-ABSORPTION-SPECTROSCOPY; PHOTOEXCITED HYDRATED ELECTRON; MONTE-CARLO CALCULATIONS; EXCITED RYDBERG ATOMS; DOPED WATER CLUSTERS; DIPOLE-BOUND ANIONS; TO-SOLVENT-STATES C1 [Young, Ryan M.; Neumark, Daniel M.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Neumark, Daniel M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Chem Sci Div, Berkeley, CA 94720 USA. RP Neumark, DM (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM dneumark@berkeley.edu RI Neumark, Daniel/B-9551-2009; OI Neumark, Daniel/0000-0002-3762-9473; Young, Ryan/0000-0002-5108-0261 FU National Science Foundation [CHE-1011819] FX This work is supported by the National Science Foundation under Grant No. CHE-1011819. DMN thanks the many graduate students and postdoctoral fellows who carried out the work in his laboratory that is reported here, and thanks Ori Cheshnovsky and Rainer Weinkauf for very fruitful collaborations in this area of research. NR 270 TC 51 Z9 51 U1 12 U2 170 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0009-2665 EI 1520-6890 J9 CHEM REV JI Chem. Rev. PD NOV PY 2012 VL 112 IS 11 BP 5553 EP 5577 DI 10.1021/cr300042h PG 25 WC Chemistry, Multidisciplinary SC Chemistry GA 039IV UT WOS:000311239600001 PM 22742559 ER PT J AU Yu, WT Porosoff, MD Chen, JGG AF Yu, Weiting Porosoff, Marc D. Chen, Jingguang G. TI Review of Pt-Based Bimetallic Catalysis: From Model Surfaces to Supported Catalysts SO CHEMICAL REVIEWS LA English DT Review ID LOW-TEMPERATURE HYDROGENATION; DENSITY-FUNCTIONAL THEORY; X-RAY-ABSORPTION; WATER-GAS-SHIFT; PREFERENTIAL CO OXIDATION; SCANNING-TUNNELING-MICROSCOPY; ENERGY-ELECTRON DIFFRACTION; CHEMICAL-VAPOR-DEPOSITION; TRANSITION-METAL CARBIDES; SINGLE-CRYSTAL SURFACES C1 [Yu, Weiting; Porosoff, Marc D.; Chen, Jingguang G.] Univ Delaware, Dept Chem & Bimol Engn, Catalysis Ctr Energy Innovat, Newark, DE 19716 USA. [Chen, Jingguang G.] Columbia Univ, Dept Chem Engn, New York, NY 10027 USA. [Chen, Jingguang G.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. RP Chen, JGG (reprint author), Univ Delaware, Dept Chem & Bimol Engn, Catalysis Ctr Energy Innovat, Newark, DE 19716 USA. EM jgchen@udel.edu RI Yu, Weiting/F-9332-2013; Porosoff, Marc/N-2816-2015 FU Catalysis Center for Energy Innovation, an Energy Frontier Research Center; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001004] FX The authors acknowledge support from the Catalysis Center for Energy Innovation, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number DE-SC0001004. NR 405 TC 349 Z9 354 U1 66 U2 668 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0009-2665 EI 1520-6890 J9 CHEM REV JI Chem. Rev. PD NOV PY 2012 VL 112 IS 11 BP 5780 EP 5817 DI 10.1021/cr300096b PG 38 WC Chemistry, Multidisciplinary SC Chemistry GA 039IV UT WOS:000311239600007 PM 22920037 ER PT J AU Chen, M Wang, SM Zhang, JZ He, DW Zhao, YS AF Chen, Miao Wang, Shanmin Zhang, Jianzhong He, Duanwei Zhao, Yusheng TI Synthesis of Stoichiometric and Bulk CrN through a Solid-State Ion-Exchange Reaction SO CHEMISTRY-A EUROPEAN JOURNAL LA English DT Article DE chromium nitride; high-pressure chemistry; ion exchange; solid-state reactions; transition metals ID CRYSTAL-STRUCTURE; HIGH-PRESSURE; COATINGS; MODULUS; TIN AB Chromium mononitride (CrN) exhibits interesting magnetic, structural, and electronic properties for technological applications. Experimental reports on these properties are often inconsistent owing to differences in the degree of nonstoichiometry in CrNx. To date, the preparation of bulk and stoichiometric CrN has been challenging; most products are in the form of a thin film produced by non-equilibrium processes, and are often nonstoichiometric and poorly crystallized. In this work, we formulated a solid-state ion-exchange route for the synthesis of CrN under high pressure. The final CrN product is phase-pure, stoichiometric, and well-crystallized in the bulk form. Near-stoichiometric and well-crystallized CrN can be synthesized using the same route at atmospheric pressure, making massive and industrial-scale production technologically feasible. The successful synthesis of stoichiometric and bulk CrN is expected to open new opportunities in diverse areas of fundamental research. C1 [Chen, Miao; Wang, Shanmin; He, Duanwei] Sichuan Univ, Inst Atom & Mol Phys, Chengdu 610065, Peoples R China. [Wang, Shanmin; Zhang, Jianzhong; Zhao, Yusheng] Los Alamos Natl Lab, LANSCE Div, Los Alamos, NM 87545 USA. [Zhao, Yusheng] Univ Nevada, HiPSEC, Las Vegas, NV 89154 USA. RP Wang, SM (reprint author), Sichuan Univ, Inst Atom & Mol Phys, Chengdu 610065, Peoples R China. EM ShanminWang@gmail.com; DuanweiHe@scu.edu.cn; Yusheng.Zhao@unlv.edu OI Zhang, Jianzhong/0000-0001-5508-1782 FU U.S. Department of Energy's Office of Basic Energy Sciences; China 973 Program [2011CB808205]; National Natural Science Foundation of China [11027405] FX This work has partly benefited from the use of the Lujan Neutron Scattering Center at Los Alamos Neutron Science Center, which is funded by the U.S. Department of Energy's Office of Basic Energy Sciences. This work is also supported by the China 973 Program (Grant No. 2011CB808205), and the National Natural Science Foundation of China (Grant No. 11027405). NR 30 TC 14 Z9 16 U1 4 U2 42 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 0947-6539 J9 CHEM-EUR J JI Chem.-Eur. J. PD NOV PY 2012 VL 18 IS 48 BP 15459 EP 15463 DI 10.1002/chem.201202197 PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA 040FF UT WOS:000311306700031 PM 23059561 ER PT J AU Hanifi, D Pun, A Liu, Y AF Hanifi, David Pun, Andrew Liu, Yi TI Synthesis and Properties of Bisphosphole-Bridged Ladder Oligophenylenes SO CHEMISTRY-AN ASIAN JOURNAL LA English DT Review DE free-radical phosphanylation; fluorescence; heteroacenes; organic semiconductors; phospholes ID PI-CONJUGATED SYSTEMS; THIN-FILM TRANSISTORS; FIELD-EFFECT TRANSISTORS; CLEAN REACTION STRATEGY; ELECTROCHEMICAL PROPERTIES; MEDIATED CYCLIZATION; ORGANIC ELECTRONICS; CATALYZED SYNTHESIS; MODEL COMPOUNDS; BUILDING-BLOCK AB Ladder-type oligophenylenes (LOPP) with bridging heteroatoms are interesting systems as they offer novel electronic and photophysical properties on account of the rigid structural features, more efficient electron delocalization on the coplanar aromatic framework, and strong intermolecular interactions. LOPPs incorporating multiple phosphorous centers combine the excellent electronic properties of phospholes and rigidified conjugated framework of LOPPs, thus positioning themselves as an attractive class of organic semiconductors. To date, there still lacks an effective synthetic methodology towards LOPPs with multiple phosphorous bridges. Herein, we describe the synthesis and properties of a new class of bisphosphole-bridged ladder oligo(p-phenylene)s and the related phosphoxides. The synthesis of phospholes was achieved by a four-fold free-radical phosphanylation reaction of a tetrabromo p-terphenylene or biphenyl-thiophene. Sequential trapping of four highly reactive aryl radicals occurred effectively to give the desired phosphorous-containing ladder compound. The oxides of the phospholes are shown to be strong fluorophores that can be used as potential n-type building blocks for organic semiconducting materials. C1 [Hanifi, David; Pun, Andrew; Liu, Yi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. RP Liu, Y (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM yliu@lbl.gov RI Liu, yi/A-3384-2008; Foundry, Molecular/G-9968-2014; OI Liu, yi/0000-0002-3954-6102; Pun, Andrew/0000-0002-3052-912X FU Office of Science, Office of Basic Energy Sciences, Scientific User Facilities Division, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was performed at the Molecular Foundry, Lawrence Berkeley National Laboratory, supported by the Office of Science, Office of Basic Energy Sciences, Scientific User Facilities Division, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 101 TC 16 Z9 16 U1 2 U2 55 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1861-4728 EI 1861-471X J9 CHEM-ASIAN J JI Chem.-Asian J. PD NOV PY 2012 VL 7 IS 11 BP 2615 EP 2620 DI 10.1002/asia.201200631 PG 6 WC Chemistry, Multidisciplinary SC Chemistry GA 019DM UT WOS:000309717300022 PM 22945900 ER PT J AU Paul, BK Hires, CL Su, YW Chang, CH Rarnprasad, S Palo, D AF Paul, B. K. Hires, C. L. Su, Y. -W. Chang, C. -H. Rarnprasad, S. Palo, D. TI A Uniform Residence Time Flow Cell for the Microreactor-Assisted Solution Deposition of CdS on an FTO-Glass Substrate SO CRYSTAL GROWTH & DESIGN LA English DT Article ID CHEMICAL BATH DEPOSITION; FILM SOLAR-CELLS; OPTIMAL-DESIGN; GEOMETRIES; CHAMBER AB Photovoltaic cells have long been a desirable alternative to the consumption of fossil fuels, but current manufacturing practices suffer from poor energy efficiency, large carbon footprints, low material utilization, and high processing temperatures. A critical step in production of thin film CdTe and CuInSe2 solar cells is the chemical bath deposition of a CdS thin film to serve as a "buffer layer" between the optically absorbent layer and the transparent conducting oxide. In prior work, functional CdS films were demonstrated at low temperature using a continuous flow, microreactor-assisted deposition process showing good selectivity of heterogeneous surface reactions over homogeneous bulk precipitation. In this paper, we develop a flow cell for implementing a uniform CdS film over a 152 mm substrate. Analytical models are coupled with computational fluid dynamic simulations to design a flow cell with more uniform flow fields. Experimental results demonstrate a 12% coefficient of variance for a 21.5 nm thick film. C1 [Paul, B. K.; Hires, C. L.] Oregon State Univ, Oregon Proc Innovat Ctr, Microprod Breakthrough Inst, Sch Mech Ind & Mfg Engn, Corvallis, OR 97330 USA. [Su, Y. -W.; Chang, C. -H.] Oregon State Univ, Oregon Proc Innovat Ctr, Microprod Breakthrough Inst, Sch Chem Biol & Environm Engn, Corvallis, OR 97330 USA. [Rarnprasad, S.; Palo, D.] Pacific NW Natl Lab, Oregon Proc Innovat Ctr, Microprod Breakthrough Inst, Corvallis, OR 97330 USA. RP Paul, BK (reprint author), Oregon State Univ, Oregon Proc Innovat Ctr, Microprod Breakthrough Inst, Sch Mech Ind & Mfg Engn, Corvallis, OR 97330 USA. EM brian.paul@oregonstate.edu FU U.S. Department of Energy, Industrial Technologies Program [NT08847, DE-AC-05-RL01830]; Oregon Nanoscience and Microtechnologies Institute (ONAMI) FX The work described herein was funded by the U.S. Department of Energy, Industrial Technologies Program, through award no. NT08847, under contract DE-AC-05-RL01830. Additional funds were received from the Oregon Nanoscience and Microtechnologies Institute (ONAMI) under a matching grant to Oregon State University. The authors would like to acknowledge the support of instrumentation equipment within the Microproducts Breakthrough Institute, Corvallis, OR by the Murdock Charitable Trust (2010004). NR 19 TC 6 Z9 6 U1 1 U2 30 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1528-7483 J9 CRYST GROWTH DES JI Cryst. Growth Des. PD NOV PY 2012 VL 12 IS 11 BP 5320 EP 5328 DI 10.1021/cg300923c PG 9 WC Chemistry, Multidisciplinary; Crystallography; Materials Science, Multidisciplinary SC Chemistry; Crystallography; Materials Science GA 039IZ UT WOS:000311240100022 ER PT J AU Babarao, R Custelcean, R Hay, BP Jiang, DE AF Babarao, Ravichandar Custelcean, Radu Hay, Benjamin P. Jiang, De-en TI Computer-Aided Design of Interpenetrated Tetrahydrofuran-Functionalized 3D Covalent Organic Frameworks for CO2 Capture SO CRYSTAL GROWTH & DESIGN LA English DT Article ID CARBON-DIOXIDE CAPTURE; MOLECULAR SIMULATIONS; RETICULAR SYNTHESIS; HYDROGEN STORAGE; ADSORPTION; CATENATION; SEPARATION; CRYSTALLINE; ISOMERISM; SORPTION AB Using computer-aided design, several interpenetrated imine-linked 3D covalent organic frameworks with diamondoid structures were assembled from tetrakis-4-formylphenylsilane as the tetrahedral node, and 3R,4R-diaminotetrahydrofuran as the link. Subsequently, the adsorption capacity of CO2 in each framework was predicted using grand canonical Monte Carlo simulations. At ambient conditions, the 4-fold interpenetrated framework, with disrotatory orientation of the tetrahedral nodes and diaxial conformation of the linker, displayed the highest adsorption capacity (similar to 4.6 mmol/g). At lower pressure, the more stable 5-fold interpenetrated framework showed higher uptake due to stronger interaction of CO2 with the framework. The contribution of framework charges to CO2 uptake was found to increase as the pore size decreases. The effect of functional group was further explored by replacing the ether oxygen with the CH2 group. Although no change was observed in the 1-fold framework, the CO2 capacity at 1 bar decreased by similar to 32% in the 5-fold interpenetrated framework. This work highlights the need for a synergistic effect of a narrow pore size and a high density of ether-oxygen groups for high-capacity CO2 adsorption. C1 [Babarao, Ravichandar; Custelcean, Radu; Hay, Benjamin P.; Jiang, De-en] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. RP Custelcean, R (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. EM custelceanr@ornl.gov; jiangd@ornl.gov RI Jiang, De-en/D-9529-2011; Babarao, Ravichandar/F-5491-2012; Custelcean, Radu/C-1037-2009 OI Jiang, De-en/0000-0001-5167-0731; Custelcean, Radu/0000-0002-0727-7972 FU Laboratory Directed Research and Development Program at Oak Ridge National Laboratory; Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy FX This work was sponsored by the Laboratory Directed Research and Development Program at Oak Ridge National Laboratory, managed by UT-Battelle, LLC for the U.S. Department of Energy. B.P.H. was supported by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy. NR 57 TC 16 Z9 16 U1 7 U2 103 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1528-7483 EI 1528-7505 J9 CRYST GROWTH DES JI Cryst. Growth Des. PD NOV PY 2012 VL 12 IS 11 BP 5349 EP 5356 DI 10.1021/cg3009688 PG 8 WC Chemistry, Multidisciplinary; Crystallography; Materials Science, Multidisciplinary SC Chemistry; Crystallography; Materials Science GA 039IZ UT WOS:000311240100025 ER PT J AU Lovejoy, KS Corley, CA Cope, EK Valentine, MC Leid, JG Purdy, GM Wilkes, JS Koppisch, AT Del Sesto, RE AF Lovejoy, Katherine S. Corley, Cynthia A. Cope, Emily K. Valentine, Michael C. Leid, Jeff G. Purdy, Geraldine M. Wilkes, John S. Koppisch, Andrew T. Del Sesto, Rico E. TI Utilization of Metal Halide Species Ambiguity to Develop Amorphous, Stabilized Pharmaceutical Agents As Ionic Liquids SO CRYSTAL GROWTH & DESIGN LA English DT Article ID ACETYLSALICYLIC-ACID; TEMPERATURE; SALTS; MIXTURES; SOLVENTS; CHLORIDE; INGREDIENTS; COMPLEXES; CATALYSIS; KINETICS AB A new strategy employs amorphous melts of active pharmaceutical agents, which are formed with metal chlorides, including ZnCl2, through speciation ambiguity. The Lewis acidic, bioinorganic ionic liquid formulations improve shelf life and water solubility and eliminate issues related to crystal polymorphism. This broad-ranging approach produces thermally robust chlorometallate preparations for use as lotions, antibiofilm agents, and in situations without refrigeration. C1 [Lovejoy, Katherine S.; Purdy, Geraldine M.; Del Sesto, Rico E.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Corley, Cynthia A.; Wilkes, John S.] USAF Acad, Dept Chem, Colorado Springs, CO 80840 USA. [Cope, Emily K.; Valentine, Michael C.; Leid, Jeff G.; Koppisch, Andrew T.] No Arizona Univ, Dept Chem & Biochem, Flagstaff, AZ 86011 USA. RP Del Sesto, RE (reprint author), Los Alamos Natl Lab, Mailstop J514,POB 1663, Los Alamos, NM 87545 USA. EM klovejoy@lanl.gov; ricod@lanl.gov OI Lovejoy, Katherine/0000-0002-9606-9453 FU U.S. Department of Energy through the LANL/LDRD Program; U.S. Department of Energy through Postdoctoral Research and Development Program FX We gratefully acknowledge the support of the U.S. Department of Energy through the LANL/LDRD and Postdoctoral Research and Development Programs for this work. NR 43 TC 4 Z9 4 U1 1 U2 22 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1528-7483 J9 CRYST GROWTH DES JI Cryst. Growth Des. PD NOV PY 2012 VL 12 IS 11 BP 5357 EP 5364 DI 10.1021/cg300969u PG 8 WC Chemistry, Multidisciplinary; Crystallography; Materials Science, Multidisciplinary SC Chemistry; Crystallography; Materials Science GA 039IZ UT WOS:000311240100026 ER PT J AU Yeager, JD Ramos, KJ Mack, NH Wang, HL Hooks, DE AF Yeager, John D. Ramos, Kyle J. Mack, Nathan H. Wang, Hsing-Lin Hooks, Daniel E. TI Transformation and Growth of Polymorphic Nuclei through Evaporative Deposition of Thin Films SO CRYSTAL GROWTH & DESIGN LA English DT Article ID FT-IR; PARACETAMOL; CRYSTALLIZATION; SOLVENT; DIVERSITY; CRYSTAL AB Rapidly dip-coating a silicon substrate in an acetaminophen solution creates a thin film of polymorphic nuclei, and the relative amounts of each polymorph vary with the type of solvent Polarized light microscopy (PLM) revealed that all films were initially amorphous and gradually crystallized over time scales of minutes to hours. Fourier transform infrared spectroscopy (FTIR) was used to identify the polymorphic form during crystallization and weeks after apparent stabilization of growth. Crystallites that initially nucleated from the amorphous films were found to be the metastable orthorhombic form. Over time, the orthorhombic crystallites stopped growing and the remaining amorphous regions transformed to the stable monoclinic form. The choice of solvent determined how fast the orthorhombic crystallites grew and thus controlled the polymorphic character of the film. For example, dip coating from an ethanol solution produced a largely orthorhombic film, while water yielded a film with mixed character. Kinetic arguments are made to discuss these results in terms of relative nucleation rates, supersaturation, and evaporation rate of the solvent We demonstrate that PLM and FTIR are suitable tools for exploring phase space with these thin films. This methodology might be applied broadly to polymorph screening and selection in evaluating pharmaceutical materials. C1 [Yeager, John D.; Ramos, Kyle J.; Mack, Nathan H.; Wang, Hsing-Lin; Hooks, Daniel E.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Yeager, JD (reprint author), MS P952 Los Alamos Natl Lab, Los Alamos, NM 87545 USA. EM jyeager@lanl.gov OI Yeager, John/0000-0002-3121-6053 FU National Nuclear Security Administration Science Campaign 2; Department of Energy/Department of Defense Joint Munitions Technology Development Program; Agnew National Security Fellowship; National Nuclear Security Administration of the U.S. Department of Energy [DE-ACS2-06NA25396] FX Funding for this work was provided by the National Nuclear Security Administration Science Campaign 2 and the Department of Energy/Department of Defense Joint Munitions Technology Development Program. J.D.Y. is supported by an Agnew National Security Fellowship. This work was performed, in part, at the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences user facility. Los Alamos National Laboratory, an affirmative action equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy under contract DE-ACS2-06NA25396. We thank D.F. Bahr (Purdue University) and D. S. Moore (LANL) for helpful discussions regarding technical content, D. Williams (LANL) for XRD measurements, and M. Wolverton (LANL) for assistance with some FTIR measurements. NR 26 TC 3 Z9 3 U1 2 U2 26 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1528-7483 J9 CRYST GROWTH DES JI Cryst. Growth Des. PD NOV PY 2012 VL 12 IS 11 BP 5513 EP 5520 DI 10.1021/cg301090t PG 8 WC Chemistry, Multidisciplinary; Crystallography; Materials Science, Multidisciplinary SC Chemistry; Crystallography; Materials Science GA 039IZ UT WOS:000311240100044 ER PT J AU Edmonds, J Calvin, K Clarke, L Kyle, P Wise, M AF Edmonds, James Calvin, Katherine Clarke, Leon Kyle, Page Wise, Marshall TI Energy and technology lessons since Rio SO ENERGY ECONOMICS LA English DT Article DE Climate change; Energy; Technology ID RESEARCH-AND-DEVELOPMENT; CO2 CONCENTRATIONS; CLIMATE; STABILIZATION; POLICY; FUTURE; NEED AB The 1992 Framework Convention on Climate Change created the basic international architecture for addressing climate change. That treaty was negotiated at a time when the research literature examining emissions mitigation and the role of energy technology was relatively limited. In the two subsequent decades a great deal has been learned. The problem of stabilizing the concentration of greenhouse gases in the atmosphere has proved far more difficult than envisioned in 1992 and the role of technology appears even more important when emissions mitigation strategies are co-developed in the context of multiple competing ends. (C) 2012 Elsevier B.V. All rights reserved. C1 [Edmonds, James; Calvin, Katherine; Clarke, Leon; Kyle, Page; Wise, Marshall] PNNL Joint Global Change Res Inst, College Pk, MD 20740 USA. RP Edmonds, J (reprint author), JGCRI, Pacific NW Natl Lab, College Pk, MD 20740 USA. EM jae@pnl.gov OI Calvin, Katherine/0000-0003-2191-4189 NR 47 TC 12 Z9 12 U1 0 U2 8 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0140-9883 J9 ENERG ECON JI Energy Econ. PD NOV PY 2012 VL 34 SU 1 BP S7 EP S14 DI 10.1016/j.eneco.2012.08.037 PG 8 WC Economics SC Business & Economics GA 044WO UT WOS:000311656100003 ER PT J AU Grisham, LR Agostinetti, P Barrera, G Blatchford, P Boilson, D Chareyre, J Chitarin, G de Esch, HPL De Lorenzi, A Franzen, P Fantz, U Gagliardi, M Hemsworth, RS Kashiwagi, M King, D Krylov, A Kuriyama, M Marconato, N Marcuzzi, D Roccella, M Rios, L Panasenkov, A Pilan, N Pavei, M Rizzolo, A Sartori, E Serianni, G Sonato, P Pilard, V Tanaka, M Tobari, H Veltri, P Zaccaria, P AF Grisham, L. R. Agostinetti, P. Barrera, G. Blatchford, P. Boilson, D. Chareyre, J. Chitarin, G. de Esch, H. P. L. De Lorenzi, A. Franzen, P. Fantz, U. Gagliardi, M. Hemsworth, R. S. Kashiwagi, M. King, D. Krylov, A. Kuriyama, M. Marconato, N. Marcuzzi, D. Roccella, M. Rios, L. Panasenkov, A. Pilan, N. Pavei, M. Rizzolo, A. Sartori, E. Serianni, G. Sonato, P. Pilard, V. Tanaka, M. Tobari, H. Veltri, P. Zaccaria, P. TI Recent improvements to the ITER neutral beam system design SO FUSION ENGINEERING AND DESIGN LA English DT Article DE Neutral beam injector; Negative ions; ITER ID NEGATIVE-ION SOURCE; RF SOURCE; SPIDER; COMPENSATION AB The ITER [1] fusion device is expected to demonstrate the feasibility of magnetically confined deuterium-tritium plasma as an energy source which might one day lead to practical power plants. Injection of energetic beams of neutral atoms (up to 1 MeV D-0 or up to 870 keV H-0) will be one of the primary methods used for heating the plasma, and for driving toroidal electrical current within it, the latter being essential in producing the required magnetic confinement field configuration. The design calls for each beamline to inject up to 16.5 MW of power through the duct into the tokamak, with an initial complement of two beamlines injecting parallel to the direction of the current arising from the tokamak transformer effect, and with the possibility of eventually adding a third beamline, also in the co-current direction. The general design of the beamlines has taken shape over the past 17 years [2], and is now predicated upon an RF-driven negative ion source based upon the line of sources developed by the Institute for Plasma Physics (IPP) at Garching during recent decades [3-5], and a multiple-aperture multiple-grid electrostatic accelerator derived from negative ion accelerators developed by the Japan Atomic Energy Agency (JAEA) across a similar span of time [6-8]. During the past years, the basic concept of the beam system has been further refined and developed, and assessment of suitable fabrication techniques has begun. While many design details which will be important to the installation and implementation of the ITER beams have been worked out during this time, this paper focuses upon those changes to the overall design concept which might be of general interest within the technical community. Published by Elsevier B.V. C1 [Grisham, L. R.] Princeton Univ, Plasma Phys Lab, Princeton, NJ 08543 USA. [Agostinetti, P.; Chitarin, G.; De Lorenzi, A.; Marconato, N.; Marcuzzi, D.; Pilan, N.; Pavei, M.; Rizzolo, A.; Sartori, E.; Serianni, G.; Sonato, P.; Veltri, P.; Zaccaria, P.] Consorzio RFX, Euratom ENEA Assoc, I-35127 Padua, Italy. [Barrera, G.; Rios, L.] EURATOM CIEMAT Assoc, Madrid 28040, Spain. [Blatchford, P.; Gagliardi, M.; King, D.] Culham Ctr Fus Energy, Abingdon OX14 3DB, Oxon, England. [Boilson, D.; Chareyre, J.; Hemsworth, R. S.; Kuriyama, M.; Pilard, V.; Tanaka, M.] ITER Org, F-13115 St Paul Les Durance, France. [de Esch, H. P. L.] CEA Cadarache, IRFM, F-13108 St Paul Les Durance, France. [Franzen, P.; Fantz, U.] Max Planck Inst Plasma Phys, EURATOM Assoc, D-85748 Garching, Germany. [Kashiwagi, M.] Japan Atom Energy Agcy, Naka, Ibaraki 3110193, Japan. [Krylov, A.; Panasenkov, A.; Tobari, H.] Russian Res Ctr, Kurchatov Inst, Moscow, Russia. [Roccella, M.] LT Calcoli SaS, I-23807 Merate, LC, Italy. RP Grisham, LR (reprint author), Princeton Univ, Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA. EM lgrisham@pppl.gov RI Chitarin, Giuseppe/H-6133-2012; OI Chitarin, Giuseppe/0000-0003-3060-8466; Sartori, Emanuele/0000-0002-5651-1825 NR 44 TC 24 Z9 24 U1 0 U2 24 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0920-3796 J9 FUSION ENG DES JI Fusion Eng. Des. PD NOV PY 2012 VL 87 IS 11 BP 1805 EP 1815 DI 10.1016/j.fusengdes.2012.08.001 PG 11 WC Nuclear Science & Technology SC Nuclear Science & Technology GA 045NB UT WOS:000311702400002 ER PT J AU Lichty, P Liang, XH Muhich, C Evanko, B Bingham, C Weimer, AW AF Lichty, Paul Liang, Xinhua Muhich, Christopher Evanko, Brian Bingham, Carl Weimer, Alan W. TI Atomic layer deposited thin film metal oxides for fuel production in a solar cavity reactor SO INTERNATIONAL JOURNAL OF HYDROGEN ENERGY LA English DT Article DE Solar thermal; Hydrogen; Atomic layer deposition; Concentrated solar reactor ID FLUIDIZED-BED REACTOR; HYDROGEN-PRODUCTION; IRON-OXIDE; WATER; DISSOCIATION; CYCLE; ZIRCONIA; FERRITES; PART AB Alumina thin film structures were produced by coating high surface area polymer particles via atomic layer deposition (ALD), using the polymer as a sacrificial template. Burnout of the polymer material left high surface area, high pore volume structures, with 15 nm wall thickness. Further deposition of up to 27 mol% Co and Fe was performed via ALD to produce high surface area CoFe2O4 particles for thermochemical water splitting. The ALD particles were thermally cycled in electrically heated lab reactors and on-sun using a concentrated solar, reflective cavity reactor. Surface area measurements of cycled ALD particles showed improved surface area retention as compared to bulk Fe2O3 nanopowders. Reaction rates as high as 15.2 and 9.8 mu mol/s/g were observed, on-sun, for H2O and CO2 splitting respectively. Thermochemical cycling in a concentrated solar cavity reactor showed an order of magnitude increase in solar utilization efficiency between ALD particles and bulk Fe2O3 nanopowders. Copyright (C) 2012, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved. C1 [Weimer, Alan W.] Univ Colorado, Dept Chem & Biol Engn, UCB, Boulder, CO 80303 USA. [Bingham, Carl] Natl Renewable Energy Lab, Golden, CO USA. RP Weimer, AW (reprint author), Univ Colorado, Dept Chem & Biol Engn, UCB, JSCBB Room C224,3415 Colorado Ave,Campus Box 596, Boulder, CO 80303 USA. EM Alan.Weimer@colorado.edu NR 19 TC 11 Z9 11 U1 2 U2 58 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-3199 EI 1879-3487 J9 INT J HYDROGEN ENERG JI Int. J. Hydrog. Energy PD NOV PY 2012 VL 37 IS 22 BP 16888 EP 16894 DI 10.1016/j.ijhydene.2012.08.004 PG 7 WC Chemistry, Physical; Electrochemistry; Energy & Fuels SC Chemistry; Electrochemistry; Energy & Fuels GA 038QF UT WOS:000311188500016 ER PT J AU Weiner, SC Fassbender, LL AF Weiner, Steven C. Fassbender, Linda L. TI Lessons learned from safety events SO INTERNATIONAL JOURNAL OF HYDROGEN ENERGY LA English DT Article DE Hydrogen safety; Incidents; Near-misses; Lessons learned AB The Hydrogen Incident Reporting and Lessons Learned website (www.h2incidents.org) was launched in 2006 as a database-driven resource for sharing lessons learned from hydrogen-related safety events to raise safety awareness and encourage knowledge-sharing. The development of this database, its first uses and subsequent enhancements have been described at the Second and Third International Conferences on Hydrogen Safety [1,2]. Since 2009, continuing work has not only highlighted the value of safety lessons learned, but enhanced how the database provides access to another safety knowledge tool, Hydrogen Safety Best Practices (http://h2bestpractices.org). Collaborations with the International Energy Agency (IEA) Hydrogen Implementing Agreement (HIA) Task 19 - Hydrogen Safety and others have enabled the database to capture safety event learning's from around the world. This paper updates recent progress, highlights the new "Lessons Learned Corner" as one means for knowledge-sharing and examines the broader potential for collecting, analyzing and using safety event information. Copyright (C) 2012, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved. C1 [Weiner, Steven C.] Pacific NW Natl Lab, Washington, DC 20024 USA. [Fassbender, Linda L.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Weiner, SC (reprint author), Pacific NW Natl Lab, 901 D St SW,Suite 900, Washington, DC 20024 USA. EM sc.weiner@pnnl.gov; linda.fassbender@pnnl.gov FU U.S. Department of Energy's Fuel Cell Technologies Program FX The authors acknowledge the technical contributions provided to the Lessons Learned Corner by Nick Barilo, Dan Dedrick, Dave Farese, Don Frikken, Andy Minister, Andy Sherman, Ed Skolnik and Matt Wilburn. We also wish to thank the U.S. Department of Energy's Fuel Cell Technologies Program (Sunita Satyapal, Program Manager; Antonio Ruiz, Safety, Codes and Standards Lead) for their support of this work. NR 6 TC 2 Z9 2 U1 1 U2 2 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-3199 J9 INT J HYDROGEN ENERG JI Int. J. Hydrog. Energy PD NOV PY 2012 VL 37 IS 22 BP 17358 EP 17363 DI 10.1016/j.ijhydene.2012.03.152 PG 6 WC Chemistry, Physical; Electrochemistry; Energy & Fuels SC Chemistry; Electrochemistry; Energy & Fuels GA 038QF UT WOS:000311188500068 ER PT J AU Ekoto, IW Houf, WG Evans, GH Merilo, EG Groethe, MA AF Ekoto, Isaac W. Houf, William G. Evans, Greg H. Merilo, Erik G. Groethe, Mark A. TI Experimental investigation of hydrogen release and ignition from fuel cell powered forklifts in enclosed spaces SO INTERNATIONAL JOURNAL OF HYDROGEN ENERGY LA English DT Article DE Dispersion; Confined ignition; Indoor refueling; Scenario analysis; Model validation ID SYSTEMS; AIR AB Due to rapid growth in the use of hydrogen powered fuel cell forklifts within warehouse enclosures, Sandia National Laboratories has worked to develop scientific methods that support the creation of new hydrogen safety codes and standards for indoor refueling operations. Based on industry stakeholder input, conducted experiments were devised to assess the utility of modeling approaches used to analyze potential consequences from ignited hydrogen leaks in facilities certified according to existing code language. Release dispersion and combustion characteristics were measured within a scaled test facility located at SRI International's Corral Hollow Test Site. Moreover, the impact of mitigation measures such as active/passive ventilation and pressure relief panels was investigated. Since it is impractical to experimentally evaluate all possible facility configurations and accident scenarios, careful characterization of the experimental boundary conditions has been performed so that collected datasets can be used to validate computational modeling approaches. Copyright (C) 2012, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved. C1 [Ekoto, Isaac W.; Houf, William G.; Evans, Greg H.] Sandia Natl Labs, Livermore, CA 94551 USA. [Merilo, Erik G.; Groethe, Mark A.] SRI Int, Menlo Pk, CA 94025 USA. RP Ekoto, IW (reprint author), Sandia Natl Labs, 7011 East Ave, Livermore, CA 94551 USA. EM iekoto@sandia.gov FU United States Department of Energy, Office of Energy Efficiency and Renewable Energy, Fuel Cell Technologies Program; U.S. DOE [DE-AC04-94-AL8500] FX This research was supported by the United States Department of Energy, Office of Energy Efficiency and Renewable Energy, Fuel Cell Technologies Program, under the Safety, Codes, and Standards subprogram element managed by Antonio Ruiz. Sandia is operated by the Sandia Corporation, a Lockheed Martin Company, for the U.S. DOE under contract No. DE-AC04-94-AL8500. NR 21 TC 6 Z9 6 U1 0 U2 11 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-3199 J9 INT J HYDROGEN ENERG JI Int. J. Hydrog. Energy PD NOV PY 2012 VL 37 IS 22 BP 17446 EP 17456 DI 10.1016/j.ijhydene.2012.03.161 PG 11 WC Chemistry, Physical; Electrochemistry; Energy & Fuels SC Chemistry; Electrochemistry; Energy & Fuels GA 038QF UT WOS:000311188500078 ER PT J AU LaChance, JL Middleton, B Groth, KM AF LaChance, Jeffrey L. Middleton, Bobby Groth, Katrina M. TI Comparison of NFPA and ISO approaches for evaluating separation distances SO INTERNATIONAL JOURNAL OF HYDROGEN ENERGY LA English DT Article DE Quantitative risk assessment; Separation distance; Hydrogen codes and standard AB The development of a set of safety codes and standards for hydrogen facilities is necessary to ensure they are designed and operated safely. To help ensure that a hydrogen facility meets an acceptable level of risk, code and standard development organizations (SDOs) are utilizing risk-informed concepts in developing hydrogen codes and standards. Two SDOs, the National Fire Protection Association (NFPA) and the International Organization for Standardization (ISO) through its Technical Committee (TC) 197 on hydrogen technologies have been developing standards for gaseous hydrogen facilities that specify the facilities have certain safety features, use equipment made of material suitable for a hydrogen environment, and have specified separation distances. Under Department of Energy funding, Sandia National Laboratories (SNL) has been supporting efforts by both of these SDOs to develop the separation distances included in their respective standards. Important goals in these efforts are to use a defensible, science-based approach to establish these requirements and to the extent possible, harmonize the requirements. International harmonization of regulations, codes and standards is critical for enabling global market penetration of hydrogen and fuel cell technologies. Copyright (C) 2012, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved. C1 [LaChance, Jeffrey L.; Middleton, Bobby; Groth, Katrina M.] Sandia Natl Labs, Albuquerque, NM 87104 USA. RP LaChance, JL (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87104 USA. EM jllacha@sandia.gov OI Groth, Katrina/0000-0002-0835-7798 NR 7 TC 1 Z9 1 U1 0 U2 2 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-3199 J9 INT J HYDROGEN ENERG JI Int. J. Hydrog. Energy PD NOV PY 2012 VL 37 IS 22 BP 17488 EP 17496 DI 10.1016/j.ijhydene.2012.05.144 PG 9 WC Chemistry, Physical; Electrochemistry; Energy & Fuels SC Chemistry; Electrochemistry; Energy & Fuels GA 038QF UT WOS:000311188500082 ER PT J AU Aceves, SM Espinosa-Loza, F Petitpas, G Ross, TO Switzer, VA AF Aceves, S. M. Espinosa-Loza, F. Petitpas, G. Ross, T. O. Switzer, V. A. TI Hydrogen safety training for laboratory researchers and technical personnel SO INTERNATIONAL JOURNAL OF HYDROGEN ENERGY LA English DT Article DE Hydrogen safety; Training; Web-based; Hands-on; Laboratory personnel AB We have developed a web-based hydrogen safety class and are developing a hands-on hydrogen safety class. The 4-h web-based class is directed to laboratory researchers who need basic hydrogen safety information (free online access at http://www.h2labsafety.org/), and it addresses hydrogen fundamentals: properties, pressure and cryogenic safety, emergency response and codes and standards. Technical operators in charge of building and testing experimental hydrogen equipment will also soon benefit from a more comprehensive 3-day hands-on safety class that will present detailed information for installation, testing and operation of hydrogen pressurized systems. The hands-on class includes a full day of classroom instruction followed by two days of laboratory work where students assemble, test and operate a pressure system based on a schematic and component description. Copyright (C) 2012, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved. C1 [Aceves, S. M.; Espinosa-Loza, F.; Petitpas, G.; Ross, T. O.; Switzer, V. A.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Aceves, SM (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave,L-792, Livermore, CA 94550 USA. EM aceves6@llnl.gov FU DOE, Office of Fuel Cell Technologies; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This project was funded by DOE, Office of Fuel Cell Technologies, Antonio Ruiz, Technology Development Manager. This work performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 5 TC 0 Z9 0 U1 1 U2 6 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-3199 J9 INT J HYDROGEN ENERG JI Int. J. Hydrog. Energy PD NOV PY 2012 VL 37 IS 22 BP 17497 EP 17501 DI 10.1016/j.ijhydene.2012.05.050 PG 5 WC Chemistry, Physical; Electrochemistry; Energy & Fuels SC Chemistry; Electrochemistry; Energy & Fuels GA 038QF UT WOS:000311188500083 ER PT J AU Buttner, WJ Burgess, R Rivkin, C Post, MB Boon-Brett, L Black, G Harskamp, F Moretto, P AF Buttner, W. J. Burgess, R. Rivkin, C. Post, M. B. Boon-Brett, L. Black, G. Harskamp, F. Moretto, P. TI Inter-laboratory assessment of hydrogen safety sensors performance under anaerobic conditions SO INTERNATIONAL JOURNAL OF HYDROGEN ENERGY LA English DT Article DE Hydrogen sensors; Hydrogen detectors; Sensing elements; Safety; Codes and standards ID RELIABILITY AB Sensors are important devices for alerting to the presence of leaked hydrogen in any application involving the production, storage, or use of hydrogen. Key missions for the sensor test laboratories in the U.S. Department of Energy, National Renewable Energy Laboratory and in the European Commission Joint Research Centre, Institute for Energy and Transport are to assure the availability and proper use of hydrogen safety sensors. As an integral element in a safety system, sensor performance should not be compromised by operational parameters. For example, safety sensors may be required to operate at reduced oxygen levels relative to air, such as that which would exist for nitrogen purges. Some sensor platforms are amenable for anaerobic operation, whereas other platforms will be deactivated and possible permanently altered with anaerobic operation. The NREL and JRC sensors laboratories assessed the ability of a number of sensor platforms to detect hydrogen under conditions of varying oxygen concentration. The performance of three common hydrogen sensor platforms, the thermal conductivity sensor, combustible gas sensor, and a palladium thin-film (metallic resistor) sensor, to operate under anaerobic conditions is presented. Copyright (C) 2012, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved. C1 [Buttner, W. J.; Burgess, R.; Rivkin, C.; Post, M. B.] Hydrogen Technol & Syst Ctr, Natl Renewable Energy Lab, Golden, CO 80401 USA. [Boon-Brett, L.; Black, G.; Harskamp, F.; Moretto, P.] European Commiss, DG Joint Res Ctr, Inst Energy & Transport, Cleaner Energy Unit, NL-1755 ZG Petten, Netherlands. RP Buttner, WJ (reprint author), Hydrogen Technol & Syst Ctr, Natl Renewable Energy Lab, 1617 Cole Blvd, Golden, CO 80401 USA. EM william.buttner@nrel.gov RI Post, Matthew/J-7528-2013 OI Post, Matthew/0000-0002-2855-8394 NR 10 TC 4 Z9 4 U1 0 U2 8 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-3199 J9 INT J HYDROGEN ENERG JI Int. J. Hydrog. Energy PD NOV PY 2012 VL 37 IS 22 BP 17540 EP 17548 DI 10.1016/j.ijhydene.2012.03.165 PG 9 WC Chemistry, Physical; Electrochemistry; Energy & Fuels SC Chemistry; Electrochemistry; Energy & Fuels GA 038QF UT WOS:000311188500089 ER PT J AU Ruggles, AJ Ekoto, IW AF Ruggles, A. J. Ekoto, I. W. TI Ignitability and mixing of underexpanded hydrogen jets SO INTERNATIONAL JOURNAL OF HYDROGEN ENERGY LA English DT Article DE Hydrogen; Choked; Notional nozzle; Ignition; Mach disc; Dispersion characteristics ID AXISYMMETRICAL TURBULENT JETS; HIGH-PRESSURE JETS; CONCENTRATION FIELD; NATURAL-GAS; BEHAVIOR; DECAY; MODEL AB Reliable methods are needed to predict ignition boundaries that result from compressed hydrogen bulk storage leaks without complex modeling. To support the development of these methods, a new high-pressure stagnation chamber has been integrated into Sandia National Laboratories' Turbulent Combustion Laboratory so that relevant compressed gas release scenarios can be replicated. For the present study, a jet with a 10:1 pressure ratio issuing from a small 0.75 mm radius nozzle has been examined. Jet exit shock structure was imaged by Schlieren photography, while quantitative Planar Laser Rayleigh Scatter imaging was used to measure instantaneous hydrogen mole fractions downstream of the Mach disk. Measured concentration statistics and ignitable boundary predictions compared favorably to analytic reconstructions of downstream jet dispersion behavior. Model results were produced from subsonic jet dispersion models and by invoking self-similarity jet scaling arguments with length scaling by experimentally measured effective source radii. Similar far field reconstructions that relied on various notional nozzle models to account for complex jet exit shock phenomena failed to satisfactorily predict the experimental findings. These results indicate further notional nozzle refinement is needed to improve the prediction fidelity. Moreover, further investigation is required to understand the effect of different pressure ratios on measured virtual origins used in the jet dispersion model. Copyright (C) 2012, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved. C1 [Ruggles, A. J.; Ekoto, I. W.] Sandia Natl Labs, Livermore, CA 94551 USA. RP Ruggles, AJ (reprint author), Sandia Natl Labs, 7011 East Ave,Bidg 905, Livermore, CA 94551 USA. EM ajruggl@sandia.gov NR 32 TC 11 Z9 12 U1 0 U2 19 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-3199 J9 INT J HYDROGEN ENERG JI Int. J. Hydrog. Energy PD NOV PY 2012 VL 37 IS 22 BP 17549 EP 17560 DI 10.1016/j.ijhydene.2012.03.063 PG 12 WC Chemistry, Physical; Electrochemistry; Energy & Fuels SC Chemistry; Electrochemistry; Energy & Fuels GA 038QF UT WOS:000311188500090 ER PT J AU Merilo, EG Groethe, MA Adamo, RC Schefer, RW Houf, WG Dedrick, DE AF Merilo, E. G. Groethe, M. A. Adamo, R. C. Schefer, R. W. Houf, W. G. Dedrick, D. E. TI Self-ignition of hydrogen releases through electrostatic discharge induced by entrained particulates SO INTERNATIONAL JOURNAL OF HYDROGEN ENERGY LA English DT Article DE Hydrogen; Self-ignition; Spontaneous ignition; Electrostatic discharge; Corona discharge; Particulates ID EXPLOSION AB The potential for particulates entrained in hydrogen releases to generate electrostatic charge and induce electrostatic discharge ignitions was investigated. A series of tests were performed in which hydrogen was released through a 3.175-mm diameter orifice from an initial pressure of 140 bar. Electrostatic field sensors were used to characterize the electrification of known quantities of iron oxide particulates deliberately entrained in the release. The ignition experiments focused on using charged particulates to induce spark discharges from isolated conductors and corona discharges. A total of 12 ignition events were observed. The results show that electrification of entrained particulates is a viable self-ignition mechanism of hydrogen releases. Copyright (C) 2012, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved. C1 [Merilo, E. G.; Groethe, M. A.; Adamo, R. C.] SRI Int, Menlo Pk, CA 94025 USA. [Schefer, R. W.; Houf, W. G.; Dedrick, D. E.] Sandia Natl Labs, Livermore, CA 94551 USA. RP Merilo, EG (reprint author), SRI Int, 333 Ravenswood Ave, Menlo Pk, CA 94025 USA. EM erik.merilo@sri.com; will@sandia.gov FU U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Hydrogen, Fuel Cells and Infrastructure Technologies Program FX This work was supported by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Hydrogen, Fuel Cells and Infrastructure Technologies Program under the Codes and Standards subprogram element managed by Antonio Ruiz. NR 23 TC 1 Z9 3 U1 2 U2 9 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-3199 J9 INT J HYDROGEN ENERG JI Int. J. Hydrog. Energy PD NOV PY 2012 VL 37 IS 22 BP 17561 EP 17570 DI 10.1016/j.ijhydene.2012.03.167 PG 10 WC Chemistry, Physical; Electrochemistry; Energy & Fuels SC Chemistry; Electrochemistry; Energy & Fuels GA 038QF UT WOS:000311188500091 ER PT J AU Ahmed, K Zhang, H Park, C AF Ahmed, K. Zhang, H. Park, C. TI NF-kB-mediated beta 1-integrin Overexpression in Radioresistance of Malignant Breast Cells in 3-Dimensional Culture SO INTERNATIONAL JOURNAL OF RADIATION ONCOLOGY BIOLOGY PHYSICS LA English DT Meeting Abstract CT 54th Annual Meeting of the American-Society-for-Radiation-Oncology (ASTRO) CY OCT 28-31, 2012 CL Boston, MA SP Amer Soc Radiat Oncol (ASTRO) C1 [Ahmed, K.; Zhang, H.; Park, C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Park, C.] Univ Calif San Francisco, San Francisco, CA 94143 USA. NR 0 TC 0 Z9 0 U1 0 U2 1 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 0360-3016 J9 INT J RADIAT ONCOL JI Int. J. Radiat. Oncol. Biol. Phys. PD NOV 1 PY 2012 VL 84 IS 3 SU S BP S126 EP S126 PG 1 WC Oncology; Radiology, Nuclear Medicine & Medical Imaging SC Oncology; Radiology, Nuclear Medicine & Medical Imaging GA 030BP UT WOS:000310542900314 ER PT J AU Nam, J Ahmed, KM Costes, S Zhang, H Sabe, H Shirato, H Park, CC AF Nam, J. Ahmed, K. M. Costes, S. Zhang, H. Sabe, H. Shirato, H. Park, C. C. TI Targeting Beta-1 Integrin Suppresses Invasive Recurrence in a 3-dimensional Model of Radiation Treated Ductal Carcinoma In situ SO INTERNATIONAL JOURNAL OF RADIATION ONCOLOGY BIOLOGY PHYSICS LA English DT Meeting Abstract CT 54th Annual Meeting of the American-Society-for-Radiation-Oncology (ASTRO) CY OCT 28-31, 2012 CL Boston, MA SP Amer Soc Radiat Oncol (ASTRO) C1 [Nam, J.; Sabe, H.; Shirato, H.] Hokkaido Univ, Grad Sch Med, Sapporo, Hokkaido 060, Japan. [Ahmed, K. M.; Costes, S.; Zhang, H.] Ernest Orlando Lawrence Berkeley Natl Lab, Berkeley, CA USA. [Park, C. C.] UCSF, Dept Radiat Oncol, San Francisco, CA USA. RI Costes, Sylvain/D-2522-2013; Sabe, Hisataka/A-4066-2012; Shirato, Hiroki/A-7068-2010 OI Costes, Sylvain/0000-0002-8542-2389; NR 0 TC 0 Z9 0 U1 0 U2 0 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 0360-3016 J9 INT J RADIAT ONCOL JI Int. J. Radiat. Oncol. Biol. Phys. PD NOV 1 PY 2012 VL 84 IS 3 SU S BP S143 EP S143 PG 1 WC Oncology; Radiology, Nuclear Medicine & Medical Imaging SC Oncology; Radiology, Nuclear Medicine & Medical Imaging GA 030BP UT WOS:000310542900355 ER PT J AU Welsh, JS AF Welsh, J. S. TI Evidence Supporting the Assertion That the Current Definition of Medical Events Is Imperfect for Prostate Permanent Implant Brachytherapy SO INTERNATIONAL JOURNAL OF RADIATION ONCOLOGY BIOLOGY PHYSICS LA English DT Meeting Abstract CT 54th Annual Meeting of the American-Society-for-Radiation-Oncology (ASTRO) CY OCT 28-31, 2012 CL Boston, MA SP Amer Soc Radiat Oncol (ASTRO) C1 [Welsh, J. S.] Fermilab Natl Accelerator Lab, NIU Neutron Therapy Facil, Batavia, IL 60510 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 0360-3016 J9 INT J RADIAT ONCOL JI Int. J. Radiat. Oncol. Biol. Phys. PD NOV 1 PY 2012 VL 84 IS 3 SU S BP S389 EP S389 PG 1 WC Oncology; Radiology, Nuclear Medicine & Medical Imaging SC Oncology; Radiology, Nuclear Medicine & Medical Imaging GA 030BP UT WOS:000310542901169 ER PT J AU Conboy, T Wright, S Pasch, J Fleming, D Rochau, G Fuller, R AF Conboy, Thomas Wright, Steven Pasch, James Fleming, Darryn Rochau, Gary Fuller, Robert TI Performance Characteristics of an Operating Supercritical CO2 Brayton Cycle SO JOURNAL OF ENGINEERING FOR GAS TURBINES AND POWER-TRANSACTIONS OF THE ASME LA English DT Article AB Supercritical CO2 (S-CO2) power cycles offer the potential for better overall plant economics due to their high power conversion efficiency over a moderate range of heat source temperatures, compact size, and potential use of standard materials in construction. Sandia National Labs (Albuquerque, NM) and the U.S. Department of Energy (DOE-NE) are in the process of constructing and operating a megawatt-scale supercritical CO2 split-flow recompression Brayton cycle with contractor Barber-Nichols Inc. (Arvada, CO). This facility can be counted among the first and only S-CO2 power producing Brayton cycles anywhere in the world. The Sandia-DOE test-loop has recently concluded a phase of construction that has substantially upgraded the facility by installing additional heaters, a second recuperating printed circuit heat exchanger (PCHE), more waste heat removal capability, higher capacity load banks, higher temperature piping, and more capable scavenging pumps to reduce windage within the turbomachinery. With these additions, the loop has greatly increased its potential for electrical power generation, and its ability to reach higher temperatures. To date, the loop has been primarily operated as a simple recuperated Brayton cycle, meaning a single turbine, single compressor, and undivided flow paths. In this configuration, the test facility has begun to realize its upgraded capacity by achieving new records in turbine inlet temperature (650 degrees F/615 K), shaft speed (52,000 rpm), pressure ratio (1.65), flow rate (2.7 kg/s), and electrical power generated (20 kWe). Operation at higher speeds, flow rates, pressures, and temperatures has allowed a more revealing look at the performance of essential power cycle components in a supercritical CO2 working fluid, including recuperation and waste heat rejection heat exchangers (PCHEs), turbines and compressors, bearings and seals, as well as auxiliary equipment. In this report, performance of these components to date will be detailed, including a discussion of expected operational limits as higher speeds and temperatures are approached. [DOI:10.1115/1.4007199] C1 [Conboy, Thomas; Wright, Steven; Pasch, James; Fleming, Darryn; Rochau, Gary] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Fuller, Robert] Barber Nichols Inc, Arvada, CO 80002 USA. RP Conboy, T (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM tmconbo@sandia.gov FU Lockheed Martin Corporation; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors would like to thank Sandia National Laboratories, the U.S. DOE-Nuclear Energy Division, Barber-Nichols Inc., and PrimeCore Systems. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 7 TC 24 Z9 24 U1 5 U2 42 PU ASME PI NEW YORK PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA SN 0742-4795 EI 1528-8919 J9 J ENG GAS TURB POWER JI J. Eng. Gas. Turbines Power-Trans. ASME PD NOV PY 2012 VL 134 IS 11 AR 111703 DI 10.1115/1.4007199 PG 12 WC Engineering, Mechanical SC Engineering GA 018MD UT WOS:000309664000011 ER PT J AU Mao, JX Nulwala, HB Luebke, DR Damodaran, K AF Mao, James X. Nulwala, Hunaid B. Luebke, David R. Damodaran, Krishnan TI Spectroscopic and computational analysis of the molecular interactions in the ionic liquid ion pair [BMP](+)[TFSI](-) SO JOURNAL OF MOLECULAR LIQUIDS LA English DT Article DE Ionic liquids; Density functional theory; [BMP](+)[TFSI](-); Infrared spectroscopy; NBO AIM ID ELECTRON-DENSITY; ENERGIES; SOLVENTS; ANION; SALT AB 1-Butyl-1-methylpyrrolidinium bis(trifluoromethylsulfonyl)imide ([BMP](+)[TFSI](-)) ion pairs were studied using DFT at the B3LYP/6-31 + G(d) level. Nine locally stable conformations of the ion pair were located. In the most stable conformation, [TFSI](-) takes a cis conformation and lies below the pyrrolidinium ring. Atoms-in-molecules (AIM) and electron density analysis indicated the existence of nine hydrogen bonds. Interaction energies were recalculated at the Second-order Moller-Plesset (MP2) level to show the importance of dispersion interaction. Further investigation through natural bond orbital (NBO) analysis provided insight into the importance of charge transfer interactions in the ion pair. Harmonic vibrations of the ion pair were calculated and compared with vibrations of the free ions as well as the experimental infrared spectrum. Assignments and frequency shifts are discussed in light of the inter-ionic interactions. (C) 2012 Elsevier B.V. All rights reserved. C1 [Mao, James X.; Damodaran, Krishnan] Univ Pittsburgh, Dept Chem, Pittsburgh, PA 15260 USA. [Nulwala, Hunaid B.; Luebke, David R.] Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. RP Damodaran, K (reprint author), Univ Pittsburgh, Dept Chem, Pittsburgh, PA 15260 USA. EM damodak@pitt.edu RI Nulwala, Hunaid/G-8126-2012 OI Nulwala, Hunaid/0000-0001-7481-3723 FU National Energy Technology Laboratory under RES [DE-FE0004000] FX This technical effort was performed in support of the National Energy Technology Laboratory's ongoing research in CO2 Capture under the RES contract DE-FE0004000. NR 41 TC 12 Z9 12 U1 3 U2 49 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-7322 J9 J MOL LIQ JI J. Mol. Liq. PD NOV PY 2012 VL 175 BP 141 EP 147 DI 10.1016/j.molliq.2012.09.001 PG 7 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 042KJ UT WOS:000311469800020 ER PT J AU Kirkpatrick, R Masiello, T Martin, M Nibler, JW Maki, A Weber, A Blake, TA AF Kirkpatrick, Robynne Masiello, Tony Martin, Matthew Nibler, Joseph W. Maki, Arthur Weber, Alfons Blake, Thomas A. TI High-resolution infrared studies of the nu(10), nu(11), nu(14), and nu(18) levels of [1.1.1]propellane SO JOURNAL OF MOLECULAR SPECTROSCOPY LA English DT Article DE Propellane; High-resolution infrared spectrum; Rovibrational constants; Coriolis interactions; Ground state structure; DFT calculations; Anharmonic frequencies ID SYMMETRIC-TOP MOLECULES; SPECTROSCOPY; PROPELLANES AB This paper is a continuation of earlier work in which the high resolution infrared spectrum of [1.1.1]propellane was measured and its k and l structure resolved for the first time. Here we present results from an analysis of more than 16000 transitions involving three fundamental bands nu(10) (E' - A'(1)), nu(11) (E' - A'(1)) nu(14) (A ''(2) A'(1)) and two difference bands (nu(10)-nu(18)) (E'-E '') and (nu(11) - nu(18)) (E' - E ''). Additional information about nu(18) was also obtained from the difference band (nu(15) + v18) - v18 (E' - E '') and the binary combination band (nu(15) + nu(18)) (E' - A'(1)). Through the use of the ground state constants reported in an earlier paper [11, rovibrational constants have been determined for all the vibrational states involved in these bands. The rovibrational parameters for the nu(18) (The rovibrational parameters for the nu(18) (E '') state were obtained from combination-differences and) state were obtained from combination-differences and showed no need to include interactions with other states. The nu(10) (E') state analysis was also straight-forward, with only a weak Coriolis interaction with the levels of the nu(14) (A) state. The latter levels are much more affected by a strong Coriolis interaction with the levels of the nearby nu(11) (E') state and also by a small but significant interaction with another state, presumably the nu(18) (E '') state, that is not directly observed. Gaussian calculations (B3LYP/cc-pVTZ) computed at the anharmonic level aided the analyses by providing initial values for many of the parameters. These theoretical results generally compare favorably with the final parameter values deduced from the spectral analyses. Finally, evidence was obtained for several level crossings between the rotational levels of the nu(11) and nu(14) states and, using a weak coupling term corresponding to a Delta k = 5, Delta/= -/+ 1 matrix element, it was possible to find transitions from the ground state that, combined with transitions to the same upper state, give a value of C-o = 0.1936515(4) cm(-1). This result, combined with the value of B-o = 0.28755833(14) cm(-1) reported earlier Ill, yields a value of 1.586277(3) A for the length of the novel axial CC bond in propellane. (C) 2012 Elsevier Inc. All rights reserved. C1 [Kirkpatrick, Robynne; Martin, Matthew; Nibler, Joseph W.] Oregon State Univ, Dept Chem, Corvallis, OR 97332 USA. [Masiello, Tony] Calif State Univ Hayward, Dept Chem & Biochem, Hayward, CA 94542 USA. [Weber, Alfons] NIST, Sensor Sci Div, Gaithersburg, MD 20899 USA. [Blake, Thomas A.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Nibler, JW (reprint author), Oregon State Univ, Dept Chem, Corvallis, OR 97332 USA. EM joseph.nibler@orst.edu FU Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory (PNNL); Battelle Memorial Institute [DE-AC05-76RLO 1830] FX R. Kirkpatrick is grateful to Oregon State University for Milton Harris, Benedict, and Shoemaker Fellowships during the course of this PhD thesis work [14]. J. Nibler acknowledges the support of the Camille and Henry Dreyfus Foundation in the form of a Senior Scientist Mentor Award. The research described here was performed, in part, in EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory (PNNL). PNNL is operated for the United States Department of Energy by the Battelle Memorial Institute under contract DE-AC05-76RLO 1830. We thank Robert Sams for helpful advice and assistance in recording the infrared spectra of propellane in this facility, and Tim Hubler, also at PNNL, for his expert advice on synthesis techniques. NR 33 TC 2 Z9 2 U1 3 U2 9 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0022-2852 J9 J MOL SPECTROSC JI J. Mol. Spectrosc. PD NOV PY 2012 VL 281 BP 51 EP 62 DI 10.1016/j.jms.2012.09.001 PG 12 WC Physics, Atomic, Molecular & Chemical; Spectroscopy SC Physics; Spectroscopy GA 046NH UT WOS:000311771200010 ER PT J AU Calo, C Lacatena, V Dhuey, SD Cabrini, S Babin, S Peroz, C Koshelev, A Ivonin, I Goltsov, A Yankov, V AF Calo, Cosimo Lacatena, Valeria Dhuey, Scott D. Cabrini, Stefano Babin, Sergey Peroz, Christophe Koshelev, Alexander Ivonin, Igor Goltsov, Alexander Yankov, Vladimir TI Fabrication of digital planar holograms into high refractive index waveguide core for spectroscopy-on-chip applications SO JOURNAL OF VACUUM SCIENCE & TECHNOLOGY B LA English DT Article ID GRATINGS; MICROSPECTROMETER; SPECTROMETER; RESONATORS AB A novel class of large-bandwidth wavelength demultiplexers, based on digital planar holography for on-chip spectroscopy applications, was fabricated in high refractive index contrast SiO2/Si3N4 planar waveguides. The devices consist of computer-generated digital planar holograms (DPHs) encoding the transfer function of the demultiplexers, engraved on the core layer of the optical waveguide. An optimized fabrication process has been developed to produce DPHs with an etching depth as low as 10 nm in Si3N4. The first spectrometer devices exhibit overall bandwidths as large as 98 nm and spectral channel spacings down to 0.3 nm/channel. (C) 2012 American Vacuum Society. [http://dx.doi.org/10.1116/1.4750038] C1 [Babin, Sergey; Peroz, Christophe] aBeam Technol Inc, Castro Valley, CA 94546 USA. [Calo, Cosimo; Lacatena, Valeria; Dhuey, Scott D.; Cabrini, Stefano] Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94702 USA. [Koshelev, Alexander; Ivonin, Igor; Goltsov, Alexander; Yankov, Vladimir] Nanoopt Devices LLC, Santa Clara, CA 95054 USA. RP Peroz, C (reprint author), aBeam Technol Inc, 5286 Dunnigan Ct, Castro Valley, CA 94546 USA. EM cp@abeamtech.com RI Koshelev, Alexander/J-2574-2014; Foundry, Molecular/G-9968-2014 FU Office of Science, Office of Basic Energy Sciences, of the United States Department of Energy [DE-AC02-05CH11231]; Air Force Office of Scientific Research (AFOSR), Air Force Materiel Command, USAF [FA9550-11-C-0045] FX Work at the Molecular Foundry was supported by the Office of Science, Office of Basic Energy Sciences, of the United States Department of Energy under Contract No. DE-AC02-05CH11231. Effort was sponsored by the Air Force Office of Scientific Research (AFOSR), Air Force Materiel Command, USAF, under Grant/Contract No. FA9550-11-C-0045. NR 20 TC 1 Z9 1 U1 0 U2 13 PU A V S AMER INST PHYSICS PI MELVILLE PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA SN 1071-1023 J9 J VAC SCI TECHNOL B JI J. Vac. Sci. Technol. B PD NOV PY 2012 VL 30 IS 6 AR 06FE01 DI 10.1116/1.4750038 PG 4 WC Engineering, Electrical & Electronic; Nanoscience & Nanotechnology; Physics, Applied SC Engineering; Science & Technology - Other Topics; Physics GA 045AV UT WOS:000311667300055 ER PT J AU Chen, CW Ren, F Chi, GC Hung, SC Huang, YP Kim, J Kravchenko, II Pearton, SJ AF Chen, Chung Wei Ren, Fan Chi, Gou-Chung Hung, Sheng-Chun Huang, Y. P. Kim, Jihyun Kravchenko, Ivan I. Pearton, Stephen J. TI UV ozone treatment for improving contact resistance on graphene SO JOURNAL OF VACUUM SCIENCE & TECHNOLOGY B LA English DT Article ID LAYER GRAPHENE; MOLECULES; OXIDE; SIO2 AB Optimized UV ozone cleaning of graphene layers on SiO2/Si substrates is shown to improve contact resistance of e-beam evaporated Ti/Au contacts by three orders of magnitude (3 x 10(-6) Omega-cm(2)) compared to untreated surfaces (4 x 10(-3) Omega-cm(2)). Subsequent annealing at 300 degrees C lowers the minimum value achieved to 7 x 10(-7) Omega-cm(2). Ozone exposure beyond an optimum time (6 min in these experiments) led to a sharp increase in sheet resistance of the graphene, producing degraded contact resistance. The UV ozone treatment is a simple and effective method for producing high quality contacts to graphene. (C) 2012 American Vacuum Society. [http://dx.doi.org/10.1116/1.4754566] C1 [Chen, Chung Wei; Ren, Fan] Univ Florida, Dept Chem Engn, Gainesville, FL 32611 USA. [Chi, Gou-Chung] Natl Chiao Tung Univ, Dept Photon, Hsinchu 300, Taiwan. [Hung, Sheng-Chun] Natl Cent Univ, Opt Sci Ctr, Jhongli 320, Taiwan. [Chen, Chung Wei; Huang, Y. P.] Natl Cent Univ, Dept Phys, Jhongli 320, Taiwan. [Kim, Jihyun] Korea Univ, Dept Chem & Biol Engn, Seoul 136701, South Korea. [Kravchenko, Ivan I.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37830 USA. [Pearton, Stephen J.] Univ Florida, Dept Mat Sci & Engn, Gainesville, FL 32611 USA. RP Chen, CW (reprint author), Natl Cent Univ, Dept Phys, Jhongli 320, Taiwan. EM spear@mse.ufl.edu RI Kim, Jihyun/F-6940-2013; Kravchenko, Ivan/K-3022-2015 OI Kravchenko, Ivan/0000-0003-4999-5822 FU National Science Council of Taiwan [NSC 100-2112-M-009-018]; NSF [ECCS 0901711]; Oak Ridge National Laboratory by the Office of Basic Energy Sciences, U.S. Department of Energy FX This work was supported by the National Science Council of Taiwan under Grant No. NSC 100-2112-M-009-018, NSF contract number ECCS 0901711 monitored by Dr. Yogesh B. Gianchandani and by NSF (J.M. Zavada). A portion of this research was conducted at the Center for Nanophase Materials Sciences, which was sponsored at Oak Ridge National Laboratory by the Office of Basic Energy Sciences, U.S. Department of Energy. NR 25 TC 18 Z9 18 U1 2 U2 43 PU A V S AMER INST PHYSICS PI MELVILLE PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA SN 1071-1023 J9 J VAC SCI TECHNOL B JI J. Vac. Sci. Technol. B PD NOV PY 2012 VL 30 IS 6 AR 060604 DI 10.1116/1.4754566 PG 3 WC Engineering, Electrical & Electronic; Nanoscience & Nanotechnology; Physics, Applied SC Engineering; Science & Technology - Other Topics; Physics GA 045AV UT WOS:000311667300082 ER PT J AU Douglas, EA Stevens, J Fishgrab, K Ford, C Shul, RJ Pearton, SJ AF Douglas, Erica A. Stevens, Jeffrey Fishgrab, Kira Ford, Christine Shul, Randy J. Pearton, Stephen J. TI Low-pressure inductively coupled plasma etching of benzocyclobutene with SF6/O-2 plasma chemistry SO JOURNAL OF VACUUM SCIENCE & TECHNOLOGY B LA English DT Article ID CF4/O-2 AB Highly anisotropic features of benzocyclobutene, a promising low stress layer for microelectromechanical systems, were achieved by inductively coupled plasma (ICP) etching with fluorine/oxygen based chemistry. The effects of chamber pressure, platen power, ICP power, and SF6/O-2 relative concentration were studied on etch rate, selectivity, and sidewall morphology. Highly anisotropic features were achieved with sidewall slopes similar to 88 degrees for almost all conditions. Grass-like residue, due to redeposition of etch material, was observed under certain conditions and is shown to be dependent on pressure, ICP power, and feature dimensions. (C) 2012 American Vacuum Society. [http://dx.doi.org/10.1116/1.4758765] C1 [Douglas, Erica A.; Pearton, Stephen J.] Univ Florida, Dept Mat Sci & Engn, Gainesville, FL 32611 USA. [Douglas, Erica A.; Stevens, Jeffrey; Fishgrab, Kira; Ford, Christine; Shul, Randy J.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Douglas, EA (reprint author), Univ Florida, Dept Mat Sci & Engn, Gainesville, FL 32611 USA. RI Douglas, Erica/J-3732-2014 OI Douglas, Erica/0000-0003-1873-0223 FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors would like to thank David Henry for numerous helpful discussions. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 14 TC 6 Z9 6 U1 0 U2 8 PU A V S AMER INST PHYSICS PI MELVILLE PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA SN 1071-1023 J9 J VAC SCI TECHNOL B JI J. Vac. Sci. Technol. B PD NOV PY 2012 VL 30 IS 6 AR 06FF06 DI 10.1116/1.4758765 PG 5 WC Engineering, Electrical & Electronic; Nanoscience & Nanotechnology; Physics, Applied SC Engineering; Science & Technology - Other Topics; Physics GA 045AV UT WOS:000311667300062 ER PT J AU Gleason, AE Tiberio, RC Mao, WL Ali, S Bolme, CA Lazicki, A Bordonaro, G Treichler, J Genova, V Eggert, JH AF Gleason, Arianna E. Tiberio, Richard C. Mao, Wendy L. Ali, Suzanne Bolme, Cynthia A. Lazicki, Amy Bordonaro, Garry Treichler, John Genova, Vincent Eggert, Jon H. TI Lithographically fabricated gratings for the interferometric measurement of material shear moduli under extreme conditions SO JOURNAL OF VACUUM SCIENCE & TECHNOLOGY B LA English DT Article ID SHOCK-LOADED SOLIDS; INNER-CORE; NORMAL-MODE; ANISOTROPY; VELOCITY; IMPACT AB Electron beam lithography and photolithography were used to fabricate diffraction gratings on targets for laser-driven shock-wave experiments. This target design was used with an optical interferometric system to measure transverse wave motion of the target during dynamic (shock-wave) compression. A wedged-shaped diamond substrate and reflective grating on the sample's surface allowed detection of transverse motion. Proof of principle tests on single-crystal < 100 > Si samples gave a transverse wave speed of 5.9 km/s at 5 GPa and a shear modulus of 81 GPa. This experimental design has tremendous potential, including the possibility of measuring the shear properties of pure iron at Earth core conditions. (C) 2012 American Vacuum Society. [http://dx.doi.org/10.1116/1.4767323] C1 [Gleason, Arianna E.; Mao, Wendy L.] Stanford Univ, Geol & Environm Sci Dept, Stanford, CA 94305 USA. [Tiberio, Richard C.] Stanford Univ, Stanford Nanopatterning Ctr, Stanford, CA 94305 USA. [Ali, Suzanne] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Bolme, Cynthia A.] Los Alamos Natl Lab, Los Alamos, NM 87544 USA. [Lazicki, Amy; Eggert, Jon H.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Bordonaro, Garry; Treichler, John; Genova, Vincent] Cornell Univ, Cornell Nanofabricat Facil, Ithaca, NY 14853 USA. RP Gleason, AE (reprint author), Stanford Univ, Geol & Environm Sci Dept, Stanford, CA 94305 USA. EM ariannag@stanford.edu RI Mao, Wendy/D-1885-2009; OI Bolme, Cynthia/0000-0002-1880-271X FU Geophysics Program at NSF [EAR0738873]; National Science Foundation [ECS-0335765] FX A. Gleason and W. Mao are supported by the Geophysics Program at NSF (EAR0738873). The e-beam lithography was performed at the Stanford Nano Shared Facilities, and the photolithography was performed at the Cornell NanoScale Facility, a member of the National Nanotechnology Infrastructure Network, which is supported by the National Science Foundation (Grant No. ECS-0335765). The authors are grateful for the assistance of T. Carver at SNC, M. Skvarla at CNF, and T. Uphaus, K. Bettencourt, and P. Mirkarimi at LLNL. NR 20 TC 0 Z9 0 U1 1 U2 13 PU A V S AMER INST PHYSICS PI MELVILLE PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA SN 1071-1023 J9 J VAC SCI TECHNOL B JI J. Vac. Sci. Technol. B PD NOV PY 2012 VL 30 IS 6 AR 06F306 DI 10.1116/1.4767323 PG 6 WC Engineering, Electrical & Electronic; Nanoscience & Nanotechnology; Physics, Applied SC Engineering; Science & Technology - Other Topics; Physics GA 045AV UT WOS:000311667300011 ER PT J AU Ilg, M Weis, CD Schwartz, J Persaud, A Ji, Q Lo, CC Bokor, J Hegyi, A Guliyev, E Rangelow, IW Schenkel, T AF Ilg, Michael Weis, Christoph D. Schwartz, Julian Persaud, Arun Ji, Qing Lo, Cheuk Chi Bokor, Jeffrey Hegyi, Alex Guliyev, Elshad Rangelow, Ivo W. Schenkel, Thomas TI Improved single ion implantation with scanning probe alignment SO JOURNAL OF VACUUM SCIENCE & TECHNOLOGY B LA English DT Article ID SILICON AB Single dopant atoms can affect transport properties in scaled semiconductor devices and coherent control of spin and charge degrees of freedom of single dopant atoms promises to enable quantum computing. The authors report on an improved technique for deterministic placement of single dopant atoms by single ion implantation with scanning probe alignment. Ions are generated in a microwave driven ion source, mass analyzed in a Wien filter, and impinge on spin readout devices after alignment of the ion beam to regions of interest with a noncontact scanning force microscope. (C) 2012 American Vacuum Society. [http://dx.doi.org/10.1116/1.4767233] C1 [Ilg, Michael; Weis, Christoph D.; Schwartz, Julian; Persaud, Arun; Ji, Qing; Schenkel, Thomas] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Ion Beam Technol Grp, Berkeley, CA 94720 USA. [Ilg, Michael; Weis, Christoph D.; Schwartz, Julian; Guliyev, Elshad; Rangelow, Ivo W.] Tech Univ Ilmenau, D-98684 Ilmenau, Germany. [Lo, Cheuk Chi; Bokor, Jeffrey; Hegyi, Alex] Univ Calif Berkeley, Dept Elect Engn & Comp Sci, Berkeley, CA 94720 USA. RP Ilg, M (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Ion Beam Technol Grp, Berkeley, CA 94720 USA. RI Foundry, Molecular/G-9968-2014; Bokor, Jeffrey/A-2683-2011 FU U.S. National Security Agency [100000080295]; DARPA through the QUEST program; DOE [DE-AC02-05CH11231]; Hertz Foundation FX The authors thank the staff of the National Center for Electron Microscopy (NCEM), The Molecular Foundry, and the UC Berkeley Nanolab for their valuable help. This work was supported in part by the U.S. National Security Agency under 100000080295, by DARPA through the QUEST program and by DOE under Contract No. DE-AC02-05CH11231 (LBNL). A. H. gratefully acknowledges the support of the Hertz Foundation. NR 21 TC 7 Z9 7 U1 2 U2 29 PU A V S AMER INST PHYSICS PI MELVILLE PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA SN 1071-1023 J9 J VAC SCI TECHNOL B JI J. Vac. Sci. Technol. B PD NOV PY 2012 VL 30 IS 6 AR 06FD04 DI 10.1116/1.4767233 PG 5 WC Engineering, Electrical & Electronic; Nanoscience & Nanotechnology; Physics, Applied SC Engineering; Science & Technology - Other Topics; Physics GA 045AV UT WOS:000311667300053 ER PT J AU Jarro, CA Donev, EU Menguc, MP Hastings, JT AF Jarro, Carlos A. Donev, Eugenii U. Menguc, Mostafa Pinar Hastings, Jeffrey Todd TI Silver patterning using an atomic force microscope tip and laser-induced chemical deposition from liquids SO JOURNAL OF VACUUM SCIENCE & TECHNOLOGY B LA English DT Article ID FIELD ENHANCEMENT; AG NANOPARTICLES; PHOTOREDUCTION; PROBE; GLASS; LITHOGRAPHY; FABRICATION; PARTICLES; GROWTH AB This article presents a new direct patterning technique in which laser photoreduction of silver from a liquid is controlled by a scanning atomic force microscope tip. Contrary to expectations, the tip suppresses, rather than enhances, deposition on the underlying substrate, and this suppression persists in the absence of the tip. Experiments presented here exclude three potential mechanisms: purely mechanical material removal, depletion of the silver precursor, and preferential photoreduction on existing deposits. These results represent a first step toward direct, negative tone, tip-based patterning of functional materials. (C) 2012 American Vacuum Society. [http://dx.doi.org/10.1116/1.4764093] C1 [Jarro, Carlos A.; Donev, Eugenii U.; Hastings, Jeffrey Todd] Univ Kentucky, Dept Elect & Comp Engn, Lexington, KY 40506 USA. [Menguc, Mostafa Pinar] Univ Kentucky, Dept Mech Engn, Lexington, KY 40506 USA. [Donev, Eugenii U.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Menguc, Mostafa Pinar] Ozyegin Univ, Ctr Energy Environm & Econ, Istanbul, Turkey. RP Jarro, CA (reprint author), Univ Kentucky, Dept Elect & Comp Engn, Lexington, KY 40506 USA. EM hastings@engr.uky.edu RI Menguc, Pinar/O-3114-2013 FU Center for Nanoscale Science and Engineering (infrastructure established under NSF) [EPS-0447479]; National Science Foundation [CMMI-0800658] FX The authors thank Greg Schardein for taking the EDS spectra and Gazi M. Huda for his valuable comments and suggestions. Experiments described here were conducted in part in the Center for Nanoscale Science and Engineering (infrastructure established under NSF Grant No. EPS-0447479) and Electron Microscopy Center at the University of Kentucky. This work was supported by the National Science Foundation under Grant No. CMMI-0800658. NR 30 TC 1 Z9 1 U1 2 U2 18 PU A V S AMER INST PHYSICS PI MELVILLE PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA SN 1071-1023 J9 J VAC SCI TECHNOL B JI J. Vac. Sci. Technol. B PD NOV PY 2012 VL 30 IS 6 AR 06FD02 DI 10.1116/1.4764093 PG 6 WC Engineering, Electrical & Electronic; Nanoscience & Nanotechnology; Physics, Applied SC Engineering; Science & Technology - Other Topics; Physics GA 045AV UT WOS:000311667300051 ER PT J AU Mankos, M Shadman, K N'Diaye, AT Schmid, AK Persson, HHJ Davis, RW AF Mankos, Marian Shadman, Khashayar N'Diaye, Alpha T. Schmid, Andreas K. Persson, Henrik H. J. Davis, Ronald W. TI Progress toward an aberration-corrected low energy electron microscope for DNA sequencing and surface analysis SO JOURNAL OF VACUUM SCIENCE & TECHNOLOGY B LA English DT Article ID LITHOGRAPHY; PRINCIPLES; MIRROR; OPTICS AB Monochromatic, aberration-corrected, dual-beam low energy electron microscopy (MAD-LEEM) is a novel imaging technique aimed at high resolution imaging of macromolecules, nanoparticles, and surfaces. MAD-LEEM combines three innovative electron-optical concepts in a single tool: a monochromator, a mirror aberration corrector, and dual electron beam illumination. The monochromator reduces the energy spread of the illuminating electron beam, which significantly improves spectroscopic and spatial resolution. The aberration corrector is needed to achieve subnanometer resolution at landing energies of a few hundred electronvolts. The dual flood illumination approach eliminates charging effects generated when a conventional, single-beam LEEM is used to image insulating specimens. The low landing energy of electrons in the range of 0 to a few hundred electronvolts is also critical for avoiding radiation damage, as high energy electrons with kilo-electron-volt kinetic energies cause irreversible damage to many specimens, in particular biological molecules. The performance of the key electron-optical components of MAD-LEEM, the aberration corrector combined with the objective lens and a magnetic beam separator, was simulated. Initial results indicate that an electrostatic electron mirror has negative spherical and chromatic aberration coefficients that can be tuned over a large parameter range. The negative aberrations generated by the electron mirror can be used to compensate the aberrations of the LEEM objective lens for a range of electron energies and provide a path to achieving subnanometer spatial resolution. First experimental results on characterizing DNA molecules immobilized on Au substrates in a LEEM are presented. Images obtained in a spin-polarized LEEM demonstrate that high contrast is achievable at low electron energies in the range of 1-10 eV and show that small changes in landing energy have a strong impact on the achievable contrast. The MAD-LEEM approach promises to significantly improve the performance of a LEEM for a wide range of applications in the biosciences, material sciences, and nanotechnology where nanometer scale resolution and analytical capabilities are required. In particular, the microscope has the potential of delivering images of unlabeled DNA strands with nucleotide-specific contrast. This simplifies specimen preparation and significantly eases the computational complexity needed to assemble the DNA sequence from individual reads. (C) 2012 American Vacuum Society. [http://dx.doi.org/10.1116/1.4764095] C1 [Mankos, Marian; Shadman, Khashayar] Electron Opt Inc, Palo Alto, CA 94303 USA. [N'Diaye, Alpha T.; Schmid, Andreas K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, NCEM, Berkeley, CA 94720 USA. [Persson, Henrik H. J.; Davis, Ronald W.] Stanford Univ, Sch Med, Stanford Genome Technol Ctr, Palo Alto, CA 94304 USA. RP Mankos, M (reprint author), Electron Opt Inc, 1000 Elwell Court 110, Palo Alto, CA 94303 USA. EM marian@electronoptica.com RI Foundry, Molecular/G-9968-2014 FU National Human Genome Research Institute (NHGRI) [R43HG006303]; Office of Science, Office of Basic Energy Sciences, Scientific User Facilities Division, of the U.S. Department of Energy [DE-AC02-05CH11231]; Alexander von Humboldt Foundation FX The authors would like to thank T. H. P. Chang for his continuous support and numerous suggestions leading to this paper. They would also like to thank Eric Munro and John Rouse of MEBS Ltd. (London, UK) for their support and fruitful discussions. This project was supported by Grant Number R43HG006303 from the National Human Genome Research Institute (NHGRI). The content is solely the responsibility of the authors and does not necessarily represent the official views of the NHGRI or the National Institutes of Health. LEEM imaging was performed at the National Center for Electron Microscopy, Lawrence Berkeley National Laboratory, and was supported by the Office of Science, Office of Basic Energy Sciences, Scientific User Facilities Division, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. A.T.N. acknowledges support from the Alexander von Humboldt Foundation. NR 33 TC 2 Z9 2 U1 0 U2 28 PU A V S AMER INST PHYSICS PI MELVILLE PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA SN 1071-1023 J9 J VAC SCI TECHNOL B JI J. Vac. Sci. Technol. B PD NOV PY 2012 VL 30 IS 6 AR 06F402 DI 10.1116/1.4764095 PG 12 WC Engineering, Electrical & Electronic; Nanoscience & Nanotechnology; Physics, Applied SC Engineering; Science & Technology - Other Topics; Physics GA 045AV UT WOS:000311667300015 PM 23847748 ER PT J AU Ocola, LE Joshi-Imre, A Kessel, C Chen, B Park, J Gosztola, D Divan, R AF Ocola, Leonidas E. Joshi-Imre, Alexandra Kessel, Cynthia Chen, Brian Park, Jonathan Gosztola, David Divan, Ralu TI Growth characterization of electron-beam-induced silver deposition from liquid precursor SO JOURNAL OF VACUUM SCIENCE & TECHNOLOGY B LA English DT Article ID MICROSCOPY; TIO2; PMMA AB Deposits of aggregated silver particles were grown from aqueous silver-nitrate solution by electron-beam induced deposition in a liquid cell in a scanning electron microscope. Electron energies of 2, 5, and 20 keV were evaluated and found to produce distinguishably different deposits. Optimal energies exist for maximum growth rate and for minimum feature sizes. The physical structure of the deposits was found to evolve with increasing thickness as silver particles grow larger and develop more structure. Optical absorbance measurements and Raman spectroscopy on adsorbed dye suggest appropriate silver purity for using this fabrication method in nano-optics applications. (C) 2012 American Vacuum Society. [http://dx.doi.org/10.1116/1.4765629] C1 [Ocola, Leonidas E.; Joshi-Imre, Alexandra; Gosztola, David; Divan, Ralu] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Kessel, Cynthia] George Washington Middle Sch, Lyons, IL 60534 USA. [Chen, Brian] Illinois Math & Sci Acad, Aurora, IL 60506 USA. [Park, Jonathan] Northwestern Univ, Dept Mol Biosci, Evanston, IL 60208 USA. RP Ocola, LE (reprint author), Argonne Natl Lab, Ctr Nanoscale Mat, 9700 S Cass Ave, Argonne, IL 60439 USA. EM ocola@anl.gov RI Joshi-Imre, Alexandra/A-2912-2010; Gosztola, David/D-9320-2011; OI Joshi-Imre, Alexandra/0000-0002-4271-1623; Gosztola, David/0000-0003-2674-1379; Ocola, Leonidas/0000-0003-4990-1064 FU U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX The authors would like to acknowledge the help of Dr. Galyna Krylova, who provided us with the silver solution and Dr. Aiqing Chen for Raman data acquisition. They thank the discussions with the group of Professor Todd Hastings at the University of Kentucky, who have pioneered liquid-phase EBID. Use of the Center for Nanoscale Materials was supported by the U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 17 TC 9 Z9 9 U1 1 U2 15 PU A V S AMER INST PHYSICS PI MELVILLE PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA SN 1071-1023 J9 J VAC SCI TECHNOL B JI J. Vac. Sci. Technol. B PD NOV PY 2012 VL 30 IS 6 AR 06FF08 DI 10.1116/1.4765629 PG 7 WC Engineering, Electrical & Electronic; Nanoscience & Nanotechnology; Physics, Applied SC Engineering; Science & Technology - Other Topics; Physics GA 045AV UT WOS:000311667300064 ER PT J AU Perera, PN Schwartzberg, AM de Oteyza, DG Dhuey, SD Harteneck, BD Cabrini, S Olynick, DL AF Perera, Pradeep N. Schwartzberg, Adam M. de Oteyza, Dimas G. Dhuey, Scott D. Harteneck, Bruce D. Cabrini, Stefano Olynick, Deirdre L. TI Selective laser ablation of radiation exposed methyl acetoxy calix(6) arene SO JOURNAL OF VACUUM SCIENCE & TECHNOLOGY B LA English DT Article ID RESIST AB The chemical mechanism of recently discovered high resolution laser dry development of methyl acetoxy calix(6) arene is probed. This process is an alternative to wet development and allows high aspect ratio patterns to be formed in resist without pattern collapse. Using infrared, Raman, and fluorescence spectroscopies, the authors have observed a reduction of the acetoxy groups, formation of hydroxyls and extended conjugation of the system due to the cross-linking under e-beam exposed film. These changes increase the laser absorption of the resist creating species that ablates under ambient conditions. Based on these studies, the authors surmise that chemical species formed during the e-beam exposure accelerate the ablation thus setting the basis for the selective ablation. (C) 2012 American Vacuum Society. [http://dx.doi.org/10.1116/1.4767347] C1 [Perera, Pradeep N.; Schwartzberg, Adam M.; de Oteyza, Dimas G.; Dhuey, Scott D.; Harteneck, Bruce D.; Cabrini, Stefano; Olynick, Deirdre L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. RP Perera, PN (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM DLOlynick@lbl.gov RI de Oteyza, Dimas/H-5955-2013; Foundry, Molecular/G-9968-2014; perera, pradeep/I-3112-2016 OI de Oteyza, Dimas/0000-0001-8060-6819; FU Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 7 TC 0 Z9 0 U1 0 U2 5 PU A V S AMER INST PHYSICS PI MELVILLE PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA SN 1071-1023 J9 J VAC SCI TECHNOL B JI J. Vac. Sci. Technol. B PD NOV PY 2012 VL 30 IS 6 AR 06FI02 DI 10.1116/1.4767347 PG 3 WC Engineering, Electrical & Electronic; Nanoscience & Nanotechnology; Physics, Applied SC Engineering; Science & Technology - Other Topics; Physics GA 045AV UT WOS:000311667300075 ER PT J AU Ruiz, R Wan, L Lille, J Patel, KC Dobisz, E Johnston, DE Kisslinger, K Black, CT AF Ruiz, Ricardo Wan, Lei Lille, Jeffrey Patel, Kanaiyalal C. Dobisz, Elizabeth Johnston, Danvers E. Kisslinger, Kim Black, Charles T. TI Image quality and pattern transfer in directed self assembly with block-selective atomic layer deposition SO JOURNAL OF VACUUM SCIENCE & TECHNOLOGY B LA English DT Article ID SEQUENTIAL INFILTRATION SYNTHESIS; DENSITY MULTIPLICATION; COPOLYMER LITHOGRAPHY; FABRICATION; BRUSHES; ARRAYS AB Self-assembled block copolymer patterns may render more robust masks for plasma etch transfer through block-selective infiltration with metal oxides, affording opportunities for improved high contrast, high fidelity pattern transfer for sub-15 nm lithography in wafer-scale processes. However, block selective infiltration alters the self-assembled block copolymer latent image by changing feature size, duty cycle, and sidewall profile. The authors systematically investigate the effects of aluminum oxide infiltration of 27 and 41 nm pitch line/space patterns formed using polystyrene-b-poly(methyl methacrylate) block copolymers and evaluate the process compatibility with directed self assembly. The degree of image distortion depends on the amount of infiltrated material, with smaller amounts resulting in complete mask hardening and larger amounts shifting and collapsing pattern features. An attractive feature of the resulting oxide mask is the relatively smooth line edge roughness of the final transferred features into Si with a 3 sigma = 2.9 nm line edge roughness. (C) 2012 American Vacuum Society. [http://dx.doi.org/10.1116/1.4758773] C1 [Ruiz, Ricardo; Wan, Lei; Lille, Jeffrey; Patel, Kanaiyalal C.; Dobisz, Elizabeth] HGST, San Jose Res Ctr, San Jose, CA 95135 USA. [Johnston, Danvers E.; Kisslinger, Kim; Black, Charles T.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Ruiz, R (reprint author), HGST, San Jose Res Ctr, San Jose, CA 95135 USA. EM ricardo.ruiz@hgst.com RI Kisslinger, Kim/F-4485-2014; OI Ruiz, Ricardo/0000-0002-1698-4281 FU U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX Research was carried out in part at the Center for Functional Nanomaterials, Brookhaven National Laboratory, which was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. NR 28 TC 26 Z9 26 U1 1 U2 59 PU A V S AMER INST PHYSICS PI MELVILLE PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA SN 1071-1023 J9 J VAC SCI TECHNOL B JI J. Vac. Sci. Technol. B PD NOV PY 2012 VL 30 IS 6 AR 06F202 DI 10.1116/1.4758773 PG 6 WC Engineering, Electrical & Electronic; Nanoscience & Nanotechnology; Physics, Applied SC Engineering; Science & Technology - Other Topics; Physics GA 045AV UT WOS:000311667300002 ER PT J AU Urbanski, L Li, W Rocca, JJ Menoni, CS Marconi, MC Isoyan, A Stein, A AF Urbanski, Lukasz Li, Wei Rocca, Jorge J. Menoni, Carmen S. Marconi, Mario C. Isoyan, Artak Stein, Aaron TI Defect tolerant extreme ultraviolet lithography technique SO JOURNAL OF VACUUM SCIENCE & TECHNOLOGY B LA English DT Article ID X-RAY LASER; INTERFERENCE NANOLITHOGRAPHY; FABRICATION AB A defect tolerant method of printing periodic structures with submicron resolution is presented. This technique is based on the self-imaging effect produced when a periodic semi-transparent mask is illuminated with coherent light. An analytical description of the effect, numerical simulations, and experimental evidence that is in good agreement with the theoretical analysis is presented. To explore the extent of defect tolerance, masks with different defect layouts were designed and tested. (C) 2012 American Vacuum Society. [http://dx.doi.org/10.1116/1.4758758] C1 [Urbanski, Lukasz; Li, Wei; Rocca, Jorge J.; Menoni, Carmen S.; Marconi, Mario C.] Colorado State Univ, Engn Res Ctr Extreme Ultraviolet Sci & Technol, Ft Collins, CO 80563 USA. [Urbanski, Lukasz; Li, Wei; Rocca, Jorge J.; Menoni, Carmen S.; Marconi, Mario C.] Colorado State Univ, Dept Elect & Comp Engn, Ft Collins, CO 80563 USA. [Isoyan, Artak] Synopsys Inc, Hillsboro, OR 97164 USA. [Stein, Aaron] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Urbanski, L (reprint author), Colorado State Univ, Engn Res Ctr Extreme Ultraviolet Sci & Technol, Ft Collins, CO 80563 USA. EM urbanski@engr.colostate.edu OI Stein, Aaron/0000-0003-4424-5416 FU National Science Foundation [ECCS 0901806]; NSF ERC for Extreme Ultraviolet Science and Technology [EEC 0310717]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX This work was supported by the National Science Foundation, award ECCS 0901806, the NSF ERC for Extreme Ultraviolet Science and Technology, award EEC 0310717. This research was carried out in part at the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. NR 21 TC 4 Z9 4 U1 1 U2 18 PU A V S AMER INST PHYSICS PI MELVILLE PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA SN 1071-1023 J9 J VAC SCI TECHNOL B JI J. Vac. Sci. Technol. B PD NOV PY 2012 VL 30 IS 6 AR 06F502 DI 10.1116/1.4758758 PG 5 WC Engineering, Electrical & Electronic; Nanoscience & Nanotechnology; Physics, Applied SC Engineering; Science & Technology - Other Topics; Physics GA 045AV UT WOS:000311667300017 ER PT J AU Sandoz, G Isacoff, EY AF Sandoz, Guillaume Isacoff, Ehud Y. TI Remotely control the activity of endogenous ion channels by light SO M S-MEDECINE SCIENCES LA French DT News Item ID POTASSIUM CHANNELS; OPTICAL CONTROL; K+ CHANNEL; TREK-1; TRAAK C1 [Sandoz, Guillaume] Univ Nice Sophia Antipolis, CNRS, Inst Pharmacol Mol & Cellulaire, F-06560 Valbonne, France. [Sandoz, Guillaume; Isacoff, Ehud Y.] Univ Calif Berkeley, Helen Wills Neurosci Inst, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Isacoff, Ehud Y.] Univ Calif Berkeley, Biophys Grad Grp, Berkeley, CA 94720 USA. [Isacoff, Ehud Y.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Sandoz, G (reprint author), Univ Nice Sophia Antipolis, CNRS, Inst Pharmacol Mol & Cellulaire, F-06560 Valbonne, France. EM sandoz@ipmc.cnrs.fr NR 15 TC 0 Z9 0 U1 2 U2 5 PU EDP SCIENCES S A PI LES ULIS CEDEX A PA 17, AVE DU HOGGAR, PA COURTABOEUF, BP 112, F-91944 LES ULIS CEDEX A, FRANCE SN 0767-0974 J9 M S-MED SCI JI M S-Med. Sci. PD NOV PY 2012 VL 28 IS 11 BP 934 EP 937 PG 4 WC Medicine, Research & Experimental SC Research & Experimental Medicine GA 043EH UT WOS:000311525200011 PM 23171896 ER PT J AU Li, YF Yin, WJ Deng, R Chen, R Chen, J Yan, QY Yao, B Sun, HD Wei, SH Wu, T AF Li, Yongfeng Yin, Wanjian Deng, Rui Chen, Rui Chen, Jing Yan, Qingyu Yao, Bin Sun, Handong Wei, Su-Huai Wu, Tom TI Realizing a SnO2-based ultraviolet light-emitting diode via breaking the dipole-forbidden rule SO NPG ASIA MATERIALS LA English DT Article DE dipole-forbidden rule; electroluminescence; first-principles calculations; light-emitting diode; photoluminescence; Tin dioxide ID LOW-TEMPERATURE PHOTOLUMINESCENCE; SNO2 NANOWIRES; ELECTRON-AFFINITY; SOLAR-CELLS; TIN OXIDE; FILMS; DYE; NANOCRYSTALS; DEPENDENCE; CONVERSION AB Although many oxide semiconductors possess wide bandgaps in the ultraviolet (UV) regime, currently the majority of them cannot efficiently emit UV light because the band-edge optical transition is forbidden in a perfect lattice as a result of the symmetry of the band-edge states. This quantum mechanical rule severely constrains the optical applications of wide-bandgap oxides, which is also the reason why so few oxides enjoy the success of ZnO. Here, using SnO2 as an example, we demonstrate both theoretically and experimentally that UV photoluminescence and electroluminescence can be recovered and enhanced in wide-bandgap oxide thin films with 'forbidden' energy gaps by engineering their nanocrystalline structures. In our experiments, the tailored low-temperature annealing process results in a hybrid structure containing SnO2 nanocrystals in an amorphous matrix, and UV emission is observed in such hybrid SnO2 thin films, indicating that the quantum mechanical dipole-forbidden rule has been effectively overcome. Using this approach, we demonstrate the first prototypical electrically pumped UV-light-emitting diode based on nanostructured SnO2 thin films. NPG Asia Materials (2012) 4, e30; doi:10.1038/am.2012.56;published online 9 November 2012 C1 [Yin, Wanjian; Wei, Su-Huai] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Li, Yongfeng; Deng, Rui; Chen, Rui; Sun, Handong; Wu, Tom] Nanyang Technol Univ, Sch Phys & Math Sci, Div Phys & Appl Phys, Singapore 637371, Singapore. [Li, Yongfeng; Yao, Bin] Jilin Univ, State Key Lab Superhard Mat, Changchun 130023, Peoples R China. [Li, Yongfeng; Yao, Bin] Jilin Univ, Dept Phys, Changchun 130023, Peoples R China. [Deng, Rui] Changchun Univ Sci & Technol, Sch Mat Sci & Engn, Changchun, Peoples R China. [Chen, Jing; Yan, Qingyu] Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 637371, Singapore. RP Wei, SH (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM suhuai.wei@nrel.gov; tomwu@ntu.edu.sg RI Sun, Handong/A-2940-2010; Yan , Qingyu/A-2237-2011; CHEN, RUI/A-1896-2010; Yin, Wanjian/F-6738-2013; Deng, Rui/A-5546-2012; Li, Yongfeng/B-8737-2012; Wu, Tom/A-1158-2012 OI Sun, Handong/0000-0002-2261-7103; CHEN, RUI/0000-0002-0445-7847; Li, Yongfeng/0000-0002-9725-0692; Wu, Tom/0000-0003-0845-4827 FU US Department of Energy [DE-AC36-08GO28308]; National Research Foundation of Singapore FX We acknowledge support from the National Research Foundation of Singapore. The work at NREL was funded by the US Department of Energy under the Grant No. DE-AC36-08GO28308. NR 46 TC 34 Z9 34 U1 3 U2 61 PU NATURE PUBLISHING GROUP PI NEW YORK PA 75 VARICK ST, 9TH FLR, NEW YORK, NY 10013-1917 USA SN 1884-4049 J9 NPG ASIA MATER JI NPG Asia Mater. PD NOV PY 2012 VL 4 AR e30 DI 10.1038/am.2012.56 PG 6 WC Materials Science, Multidisciplinary SC Materials Science GA 048DU UT WOS:000311891200001 ER PT J AU Harrison, AK AF Harrison, Alan K. TI Calculation of the electron two-slit experiment using a quantum mechanical variational principle SO PHYSICA SCRIPTA LA English DT Article AB A nonlocal relativistic variational principle (VP) has recently been proposed as an alternative to the Dirac wave equation of standard quantum mechanics. We apply that principle to the electron two-slit experiment. The detection system is modeled as a screen made of atoms, any one of which can be excited by the incident electron, but we avoid restricting the detection mechanism further. The VP is shown to predict that, at the time the electron reaches the screen, its wavefunction will be localized to the neighborhood of a single atom, resulting in a position-type measurement. In an ensemble of such experiments ('identically prepared' except that the initial phase of the wavefunction-the hidden variable in the VP formulation-is sampled over the expected uniform distribution), the distribution of measured positions will reproduce the interference pattern predicted by the Dirac equation. We also demonstrate that with a detection system designed fundamentally to detect the electron's transverse wavelength rather than its position, the VP predicts that one such mode will be detected, that is, a wavelength measurement will result. Finally, it is shown that these results are unchanged in the 'delayed choice' variant of the experiment. C1 Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Harrison, AK (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM alanh@lanl.gov FU NNSA ASC program FX This work has been supported by the NNSA ASC program. The author appreciates support from Jerry Brock, Mark Chadwick and Robert Webster; helpful discussions with Salman Habib, Robin Blume-Kohout, Terry Goldman, Howard Brandt, Baolian Cheng and David Sigeti; review of an earlier draft by Jean-Francois Van Huele; and detailed discussions with Dale W Harrison and B Kent Harrison over a long period of time. He is, however, solely responsible for any errors or deficiencies in the work. NR 6 TC 0 Z9 0 U1 0 U2 4 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0031-8949 J9 PHYS SCRIPTA JI Phys. Scr. PD NOV PY 2012 VL T151 AR 014006 DI 10.1088/0031-8949/2012/T151/014006 PG 8 WC Physics, Multidisciplinary SC Physics GA 049DH UT WOS:000311961700007 ER PT J AU Park, JF Watson, CR Buschbom, RL Dagle, GE Strom, DJ Weller, RE AF Park, James F. Watson, Charles R. Buschbom, Ray L. Dagle, Gerald E. Strom, Daniel J. Weller, Richard E. TI Biological Effects of Inhaled (PuO2)-Pu-239 in Beagles SO RADIATION RESEARCH LA English DT Article ID GROWTH-FACTOR RECEPTOR; LUNG-TUMORS; PLUTONIUM INHALATION; DOGS; EXPOSURE; PU-239; MORTALITY; TOXICITY; AEROSOLS; DIOXIDE AB Park, J. F., Watson, C. R., Buschbom, R. L., Dagle, G. E, Strom, D. J. and Weller, R. E. Biological Effects of Inhaled (PuO2)-Pu-239 in Beagles. Radiat. Res. 178, 447-467 (2012). Seven groups of 8-24 Beagle dogs, exposed to (PuO2)-Pu-239 aerosols by inhalation [mean initial lung depositions (ILD) of 0.0, 0.14, 0.63, 3.2, 13, 44 and 210 kBq] were observed throughout their lives to determine tissues at risk and dose-effect relationships. The mean average pulmonary retention half-time of Pu-739 was 1,192 days. Most (70%) of the plutonium recovered at death in dogs surviving >10 years after exposure was found in the thoracic lymph nodes with similar to 15% in lung, similar to 10% in liver and similar to 2% in bone. Eight dogs at the highest exposure levels died from radiation pneumonitis prior to a minimal 3-year latency period after exposure for the observation of lung tumors, with the first succumbing 337 days after exposure. Of 108 plutonium-exposed Beagles with ILD <100 kBq, 51(47%) had lung tumors with significantly increased incidence in those dogs with total lung dose of >= 1.1 Gy at death. The primary non-neoplastic effects observed were lymphopenia, atrophy and fibrosis of the thoracic lymph nodes, radiation pneumonitis and pulmonary fibrosis, and bacterial pneumonia. Lesions of the thoracic lymph nodes were observed in 98 of 108 exposed dogs, but there were no primary neoplasms of the lymph nodes. Bacterial pneumonia was observed in 13 plutonium-exposed dogs and was the most notable nonneoplastic cause of death, with survival nearly the same as that of controls. Setting of dose limits on the basis of detrimental effects commonly considers and differentiates between stochastic and deterministic effects, raising the question of whether the non-neoplastic effects found in this study were deterministic. The International Commission on Radiation Protection (ICRP), National Council on Radiation Protection & Measurements (NCRP), and similar organizations generally consider effects that increase in incidence and severity to meet the definition of deterministic. We demonstrated the radiation dose-related nature of effects such as pneumonitis and fibrosis graphically and lymphopenia numerically, rather than by quantified estimates. It is clear, however, that both incidence and severity increased with ILD and radiation dose and should be considered as deterministic effects. (C) 2012 by Radiation Research Society C1 [Watson, Charles R.] Washington State Univ Tri Cities, Richland, WA USA. [Park, James F.; Buschbom, Ray L.; Dagle, Gerald E.; Strom, Daniel J.; Weller, Richard E.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Weller, RE (reprint author), 902 Battelle Blvd,K9-81, Richland, WA 99354 USA. EM dick.weller@pnl.gov OI Strom, Daniel J/0000-0002-1710-3634 FU Office of Biological and Environmental Research of the U.S. Department of Energy [DE-AC06-76RLO 1830] FX This manuscript is based on a study that was supported by the Office of Biological and Environmental Research of the U.S. Department of Energy under Contract DE-AC06-76RLO 1830. The study was conducted in facilities fully accredited by the American Association for Accreditation of Laboratory Animal Care, and according to protocols approved by the Institutional Animal Care and Use Committee. The authors accept full responsibility for summarizing and presenting the results of this study but recognize that many past and present members of Pacific Northwest National Laboratory's professional and technical staff also made significant contributions. Specifically, we thank W.J. Bair, J.M. Thomas, the late R.C. Thompson, and J.A. Mahaffey for guidance in experimental design; D.L. Craig and W.C. Cannon for aerosol generation and characterization; K.L. Swinth for in vivo counting; S.E. Rowe for veterinary medicine; E.L. Wierman for animal care; G.J. Powers for plutonium radioanalysis of tissues and excreta; H.A. Ragan for hematology and clinical chemistry measurements; and finally, the late M.R. Sikov for many thoughtful and insightful suggestions for summarizing this study. The authors also thank D.L. Felton and J.G. Wiley for editing this manuscript. Detailed records associated with this study have been transferred to the National Radiobiology Archives (NRA), operated for the Department of Energy by the Transuranium and Uranium Registries at Washington State university-Tri Cities. Electronic copies of the detailed records are available for use: direct requests to Sergei Tolmachev. NR 69 TC 3 Z9 3 U1 1 U2 11 PU RADIATION RESEARCH SOC PI LAWRENCE PA 810 E TENTH STREET, LAWRENCE, KS 66044 USA SN 0033-7587 J9 RADIAT RES JI Radiat. Res. PD NOV PY 2012 VL 178 IS 5 BP 447 EP 467 DI 10.1667/RR2504.1 PG 21 WC Biology; Biophysics; Radiology, Nuclear Medicine & Medical Imaging SC Life Sciences & Biomedicine - Other Topics; Biophysics; Radiology, Nuclear Medicine & Medical Imaging GA 044ZT UT WOS:000311664400008 PM 22998225 ER PT J AU Kung, Y Runguphan, W Keasling, JD AF Kung, Yan Runguphan, Weerawat Keasling, Jay D. TI From Fields to Fuels: Recent Advances in the Microbial Production of Biofuels SO ACS SYNTHETIC BIOLOGY LA English DT Review DE metabolic engineering; biofuels; alcohols; fatty acids; isoprenoids ID ENGINEERED ESCHERICHIA-COLI; CYANOBACTERIAL ALDEHYDE DECARBONYLASE; FATTY-ACID SYNTHASES; SACCHAROMYCES-CEREVISIAE; LYCOPENE PRODUCTION; DIRECTED EVOLUTION; MEVALONATE PATHWAY; ISOPROPANOL PRODUCTION; SYNTHETIC DESIGN; BIOSYNTHESIS AB Amid grave concerns over global climate change and with increasingly strained access to fossil fuels, the synthetic biology community has stepped up to the challenge of developing microbial platforms for the production of advanced biofuels. The adoption of gasoline, diesel, and jet fuel alternatives derived from microbial sources has the potential to significantly limit net greenhouse gas emissions. In this effort, great strides have been made in recent years toward the engineering of microorganisms to produce transportation fuels derived from alcohol, fatty acid, and isoprenoid microorganisms. We also highlight many of the commonly used and newly devised engineering strategies biosynthesis. We provide an overview of the biosynthetic pathways devised in the strain development of biofuel-producing microorganisms. We also highlight many of the commonly used and newly devised engineering strategies that have been employed to identify and overcome pathway bottlenecks and problems of toxicity to maximize production titers. C1 [Kung, Yan; Runguphan, Weerawat; Keasling, Jay D.] Joint BioEnergy Inst, Emeryville, CA 94608 USA. [Kung, Yan; Runguphan, Weerawat; Keasling, Jay D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Keasling, Jay D.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Keasling, Jay D.] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. RP Keasling, JD (reprint author), Joint BioEnergy Inst, 5885 Hollis St, Emeryville, CA 94608 USA. EM jdkeasling@lbl.gov RI Keasling, Jay/J-9162-2012 OI Keasling, Jay/0000-0003-4170-6088 FU Office of Science, Office of Biological and Environmental Research, of the U.S. Department of Energy [DE-AC02-05CH11231] FX We thank Weslee S. Glenn (Department of Chemistry, Massachusetts Institute of Technology and Department of Biological Chemistry, John Innes Centre) for his critical reading of this manuscript and Purin Panichphant for his help with figures. This work conducted by the Joint BioEnergy Institute was supported by the Office of Science, Office of Biological and Environmental Research, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231.68 NR 105 TC 37 Z9 37 U1 8 U2 213 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2161-5063 J9 ACS SYNTH BIOL JI ACS Synth. Biol. PD NOV PY 2012 VL 1 IS 11 BP 498 EP 513 DI 10.1021/sb300074k PG 16 WC Biochemical Research Methods SC Biochemistry & Molecular Biology GA 040LW UT WOS:000311325100002 PM 23656227 ER PT J AU Chou, HH Keasling, JD AF Chou, Howard H. Keasling, Jay D. TI Synthetic Pathway for Production of Five-Carbon Alcohols from Isopentenyl Diphosphate SO APPLIED AND ENVIRONMENTAL MICROBIOLOGY LA English DT Article ID KETOGLUTARATE REDUCTASE/SACCHAROPINE DEHYDROGENASE; YELLOW ENZYME FAMILY; ESCHERICHIA-COLI; SACCHAROMYCES-CEREVISIAE; KNOCKOUT STRATEGIES; MEVALONATE PATHWAY; EVOLUTION; GENE; EXPRESSION; IDENTIFICATION AB Synthetic biological pathways could enhance the development of novel processes to produce chemicals from renewable resources. On the basis of models that describe the evolution of metabolic pathways and enzymes in nature, we developed a framework to rationally identify enzymes able to catalyze reactions on new substrates that overcomes one of the major bottlenecks in the assembly of a synthetic biological pathway. We verified the framework by implementing a pathway with two novel enzymatic reactions to convert isopentenyl diphosphate into 3-methyl-3-butenol, 3-methyl-2-butenol, and 3-methylbutanol. To overcome competition with native pathways that share the same substrate, we engineered two bifunctional enzymes that redirect metabolic flux toward the synthetic pathway. Taken together, our work demonstrates a new approach to the engineering of novel synthetic pathways in the cell. C1 [Chou, Howard H.; Keasling, Jay D.] Univ Calif Berkeley, UCSF UCB Joint Grad Grp Bioengn, Berkeley, CA 94720 USA. [Chou, Howard H.; Keasling, Jay D.] Joint BioEnergy Inst, Emeryville, CA USA. [Chou, Howard H.; Keasling, Jay D.] Univ Calif Berkeley, Synthet Biol Engn Res Ctr, Berkeley, CA 94720 USA. [Keasling, Jay D.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Keasling, Jay D.] Univ Calif Berkeley, Calif Inst Quantitat Biosci, Berkeley, CA 94720 USA. [Keasling, Jay D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Keasling, JD (reprint author), Univ Calif Berkeley, UCSF UCB Joint Grad Grp Bioengn, Berkeley, CA 94720 USA. EM keasling@berkeley.edu RI Keasling, Jay/J-9162-2012 OI Keasling, Jay/0000-0003-4170-6088 FU Joint BioEnergy Institute [DE-AC02-05CH11231]; Synthetic Biology Engineering Research Center (SynBERC) through National Science Foundation [BES-0439124] FX This work was supported by the Joint BioEnergy Institute, contract DE-AC02-05CH11231 between Lawrence Berkeley National Laboratory and the U.S. Department of Energy, and by the Synthetic Biology Engineering Research Center (SynBERC) through National Science Foundation grant BES-0439124. NR 50 TC 24 Z9 25 U1 2 U2 33 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 0099-2240 J9 APPL ENVIRON MICROB JI Appl. Environ. Microbiol. PD NOV PY 2012 VL 78 IS 22 BP 7849 EP 7855 DI 10.1128/AEM.01175-12 PG 7 WC Biotechnology & Applied Microbiology; Microbiology SC Biotechnology & Applied Microbiology; Microbiology GA 028MX UT WOS:000310427500005 PM 22941086 ER PT J AU Hwang, C Ling, FQ Andersen, GL LeChevallier, MW Liu, WT AF Hwang, Chiachi Ling, Fangqiong Andersen, Gary L. LeChevallier, Mark W. Liu, Wen-Tso TI Microbial Community Dynamics of an Urban Drinking Water Distribution System Subjected to Phases of Chloramination and Chlorination Treatments SO APPLIED AND ENVIRONMENTAL MICROBIOLOGY LA English DT Article ID DISCONTINUOUS CHLORINATION; BACTERIAL COMMUNITIES; ORGANIC-MATTER; BIOFILMS; REGROWTH; RNA; DNA; POPULATIONS; DIVERSITY; PLANTS AB Water utilities in parts of the U.S. control microbial regrowth in drinking water distribution systems (DWDS) by alternating postdisinfection methods between chlorination and chloramination. To examine how this strategy influences drinking water microbial communities, an urban DWDS (population congruent to 40,000) with groundwater as the source water was studied for approximately 2 years. Water samples were collected at five locations in the network at different seasons and analyzed for their chemical and physical characteristics and for their microbial community composition and structure by examining the 16S rRNA gene via terminal restriction fragment length polymorphism and DNA pyrosequencing technology. Nonmetric multidimension scaling and canonical correspondence analysis of microbial community profiles could explain >57% of the variation. Clustering of samples based on disinfection types (free chlorine versus combined chlorine) and sampling time was observed to correlate to the shifts in microbial communities. Sampling location and water age (<21.2 h) had no apparent effects on the microbial compositions of samples from most time points. Microbial community analysis revealed that among major core populations, Cyanobacteria, Methylobacteriaceae, Sphingomonadaceae, and Xanthomonadaceae were more abundant in chlorinated water, and Methylophilaceae, Methylococcaceae, and Pseudomonadaceae were more abundant in chloraminated water. No correlation was observed with minor populations that were detected frequently (<0.1% of total pyrosequences), which were likely present in source water and survived through the treatment process. Transient microbial populations including Flavobacteriaceae and Clostridiaceae were also observed. Overall, reversible shifts in microbial communities were especially pronounced with chloramination, suggesting stronger selection of microbial populations from chloramines than chlorine. C1 [Hwang, Chiachi; Ling, Fangqiong; Liu, Wen-Tso] Univ Illinois, Dept Civil & Environm Engn, Urbana, IL USA. [Andersen, Gary L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Ecol, Div Earth Sci, Berkeley, CA 94720 USA. [LeChevallier, Mark W.] Amer Water, Voorhees, NJ USA. RP Liu, WT (reprint author), Univ Illinois, Dept Civil & Environm Engn, Urbana, IL USA. EM wtliu@illinois.edu RI Liu, Wen-Tso/C-8788-2011; Andersen, Gary/G-2792-2015 OI Liu, Wen-Tso/0000-0002-8700-9803; Andersen, Gary/0000-0002-1618-9827 FU Water Research Foundation FX This study was supported by the Water Research Foundation. NR 42 TC 40 Z9 40 U1 4 U2 71 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 0099-2240 EI 1098-5336 J9 APPL ENVIRON MICROB JI Appl. Environ. Microbiol. PD NOV PY 2012 VL 78 IS 22 BP 7856 EP 7865 DI 10.1128/AEM.01892-12 PG 10 WC Biotechnology & Applied Microbiology; Microbiology SC Biotechnology & Applied Microbiology; Microbiology GA 028MX UT WOS:000310427500006 PM 22941076 ER PT J AU Ahmed, B Cao, B McLean, JS Ica, T Dohnalkova, A Istanbullu, O Paksoy, A Fredrickson, JK Beyenal, H AF Ahmed, Bulbul Cao, Bin McLean, Jeffrey S. Ica, Tuba Dohnalkova, Alice Istanbullu, Ozlem Paksoy, Akin Fredrickson, Jim K. Beyenal, Haluk TI Fe(III) Reduction and U(VI) Immobilization by Paenibacillus sp Strain 300A, Isolated from Hanford 300A Subsurface Sediments SO APPLIED AND ENVIRONMENTAL MICROBIOLOGY LA English DT Article ID EXTRACELLULAR ELECTRON-TRANSFER; DISSIMILATORY METAL REDUCTION; URANIUM(VI) REDUCTION; MICROBIAL REDUCTION; REDUCING BACTERIUM; GEOBACTER-METALLIREDUCENS; SHEWANELLA-PUTREFACIENS; CONTAMINATED AQUIFER; ABIOTIC REDUCTION; HUMIC SUBSTANCES AB A facultative iron-reducing [Fe(III)-reducing] Paenibacillus sp. strain was isolated from Hanford 300A subsurface sediment biofilms that was capable of reducing soluble Fe(III) complexes [Fe(III)-nitrilotriacetic acid and Fe(III)-citrate] but unable to reduce poorly crystalline ferrihydrite (Fh). However, Paenibacillus sp. 300A was capable of reducing Fh in the presence of low concentrations (2 mu M) of either of the electron transfer mediators (ETMs) flavin mononucleotide (FMN) or anthraquinone-2,6-disulfonate (AQDS). Maximum initial Fh reduction rates were observed at catalytic concentrations (<10 mu M) of either FMN or AQDS. Higher FMN concentrations inhibited Fh reduction, while increased AQDS concentrations did not. We also found that Paenibacillus sp. 300A could reduce Fh in the presence of natural ETMs from Hanford 300A subsurface sediments. In the absence of ETMs, Paenibacillus sp. 300A was capable of immobilizing U(VI) through both reduction and adsorption. The relative contributions of adsorption and microbial reduction to U(VI) removal from the aqueous phase were similar to 7:3 in PIPES [piperazine-N, N'-bis(2-ethanesulfonic acid)] and similar to 1:4 in bicarbonate buffer. Our study demonstrated that Paenibacillus sp. 300A catalyzes Fe(III) reduction and U(VI) immobilization and that these reactions benefit from externally added or naturally existing ETMs in 300A subsurface sediments. C1 [Ahmed, Bulbul; Cao, Bin; Ica, Tuba; Istanbullu, Ozlem; Paksoy, Akin; Beyenal, Haluk] Washington State Univ, Gene & Linda Voiland Sch Chem Engn, Pullman, WA 99164 USA. [Cao, Bin; Dohnalkova, Alice; Fredrickson, Jim K.] Pacific NW Natl Lab, Richland, WA 99352 USA. [McLean, Jeffrey S.] J Craig Venter Inst, San Diego, CA USA. [Ica, Tuba] Dumlupinar Univ, Fac Art & Sci, Dept Biol, Kutahya, Turkey. RP Beyenal, H (reprint author), Washington State Univ, Gene & Linda Voiland Sch Chem Engn, Pullman, WA 99164 USA. EM beyenal@wsu.edu RI Cao, Bin/H-2639-2012; McLean, Jeffrey/A-8014-2012 OI Cao, Bin/0000-0002-9462-496X; McLean, Jeffrey/0000-0001-9934-5137 FU U.S. DOE Office of Biological and Environmental Research under the Subsurface Biogeochemistry Research (SBR) Program [DE-FG92-08ER64560]; DOE-BER SBR Program's Scientific Focus Area (SFA) at the Pacific Northwest National Laboratory (PNNL); DOE's Office of Biological and Environmental Research and located at PNNL; DOE [DE-AC05-76RL01830] FX This research was supported by the U.S. DOE Office of Biological and Environmental Research under the Subsurface Biogeochemistry Research (SBR) Program (grant DE-FG92-08ER64560) and the DOE-BER SBR Program's Scientific Focus Area (SFA) at the Pacific Northwest National Laboratory (PNNL). We are also grateful to the Franceschi Microscopy and Imaging Center of Washington State University for the use of their facilities and for staff assistance.; A portion of the research was performed in the William R. Wiley Environmental Molecular Sciences Laboratory, a national scientific user facility sponsored by the DOE's Office of Biological and Environmental Research and located at PNNL. PNNL is operated by Battelle for the DOE under contract DE-AC05-76RL01830. NR 74 TC 5 Z9 5 U1 3 U2 45 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 0099-2240 J9 APPL ENVIRON MICROB JI Appl. Environ. Microbiol. PD NOV PY 2012 VL 78 IS 22 BP 8001 EP 8009 DI 10.1128/AEM.01844-12 PG 9 WC Biotechnology & Applied Microbiology; Microbiology SC Biotechnology & Applied Microbiology; Microbiology GA 028MX UT WOS:000310427500023 PM 22961903 ER PT J AU Oztoprak, BG Gonzalez, J Yoo, J Gulecen, T Mutlu, N Russo, RE Gundogdu, O Demir, A AF Oztoprak, Belgin Genc Gonzalez, Jhanis Yoo, Jong Gulecen, Turgay Mutlu, Nazim Russo, Richard E. Gundogdu, Ozcan Demir, Arif TI Analysis and Classification of Heterogeneous Kidney Stones Using Laser-Induced Breakdown Spectroscopy (LIBS) SO APPLIED SPECTROSCOPY LA English DT Article DE Laser-induced breakdown spectroscopy; LIBS; Kidney stone; X-ray diffraction; XRD; X-ray fluorescence; XRF; Principal component analysis; PCA; Partial least squares discrimination analysis; PLS-DA ID INDUCED PLASMA SPECTROSCOPY; ELEMENTAL ANALYSIS; URINARY CALCULI; IDENTIFICATION; COPPER; ZINC AB Kidney stones were analyzed using laser-induced breakdown spectroscopy (LIBS), utilizing a high resolution multi-channel charge-coupled device (CCD) spectrometer and a nanosecond-pulse Nd : YAG laser. The kidney stones were also characterized using X-ray diffraction (XRD) and X-ray fluorescence (XRF) techniques for comparative analysis. It was found that the ratio of hydrogen (H) to carbon (C) was an important indicator of organic compounds such as uric acid. Advantages of LIBS, especially with regards to amount of sample required and sample preparation as well as the ability to carry out elemental analysis and classification of kidney stones simultaneously, over other analytical techniques such as XRD and XRF are discussed. The common minor elements detected in the kidney stones include P, S, Si, Ti, and Zn. Principal component analysis (PCA) and partial least squares discriminant analysis (PLS-DA) of broadband LIBS spectra were employed for classifying different types of kidney stones. The results are beneficial in understanding kidney stone formation processes, which can lead to preventive therapeutic strategies and treatment methods for urological patients. C1 [Gundogdu, Ozcan; Demir, Arif] Kocaeli Univ, Inst Nat Sci, Dept Electroopt Syst Engn, TR-41380 Kocaeli, Turkey. [Oztoprak, Belgin Genc] Kocaeli Univ, Laser Technol Res & Applicat Ctr, TR-41275 Kocaeli, Turkey. [Gonzalez, Jhanis; Yoo, Jong] Appl Spectra Inc, Fremont, CA 94558 USA. [Gulecen, Turgay; Mutlu, Nazim] Kocaeli Univ, Fac Med, Dept Urol, TR-41380 Kocaeli, Turkey. [Russo, Richard E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Oztoprak, Belgin Genc] BEAM Ar Ge Opt Laser & Spect, TR-41275 Kocaeli, Turkey. RP Demir, A (reprint author), Kocaeli Univ, Inst Nat Sci, Dept Electroopt Syst Engn, TR-41380 Kocaeli, Turkey. EM arifd@kocaeli.edu.tr FU State Planning Organization of Turkey [2011K120330]; Kocaeli University [2010/96]; Ministry of Science, Industry and Technology of Turkey [404.TGSD.2010] FX This work is supported by the State Planning Organization of Turkey, Kocaeli University Research Fund, and the Ministry of Science, Industry and Technology of Turkey under contracts 2011K120330, 2010/96 and 404.TGSD.2010 projects, respectively. NR 35 TC 15 Z9 15 U1 4 U2 41 PU SOC APPLIED SPECTROSCOPY PI FREDERICK PA 5320 SPECTRUM DRIVE SUITE C, FREDERICK, MD 21703 USA SN 0003-7028 J9 APPL SPECTROSC JI Appl. Spectrosc. PD NOV PY 2012 VL 66 IS 11 BP 1353 EP 1361 DI 10.1366/12-06679 PG 9 WC Instruments & Instrumentation; Spectroscopy SC Instruments & Instrumentation; Spectroscopy GA 039TC UT WOS:000311268400013 PM 23146192 ER PT J AU Ponoum, R Cooperman, A Brodrick, J AF Ponoum, Ratcharit Cooperman, Alissa Brodrick, James TI Cloud-Based BEMS SO ASHRAE JOURNAL LA English DT Editorial Material C1 [Brodrick, James] US DOE, Bldg Technol Program, Washington, DC USA. NR 13 TC 0 Z9 0 U1 0 U2 1 PU AMER SOC HEATING REFRIGERATING AIR-CONDITIONING ENG, INC, PI ATLANTA PA 1791 TULLIE CIRCLE NE, ATLANTA, GA 30329 USA SN 0001-2491 J9 ASHRAE J JI ASHRAE J. PD NOV PY 2012 VL 54 IS 11 BP 68 EP 70 PG 3 WC Thermodynamics; Construction & Building Technology; Engineering, Mechanical SC Thermodynamics; Construction & Building Technology; Engineering GA 039TE UT WOS:000311268600019 ER PT J AU Holmberg, DG Ghatikar, G Koch, EL Boch, J AF Holmberg, David G. Ghatikar, Girish Koch, Edward L. Boch, Jim TI OpenADR Advances SO ASHRAE JOURNAL LA English DT Article C1 [Holmberg, David G.] NIST, Mech Syst & Controls Grp, Div Energy & Environm, Engn Lab, Gaithersburg, MD 20899 USA. [Ghatikar, Girish] US DOE, Lawrence Berkeley Natl Lab, Washington, DC 20585 USA. [Boch, Jim] IPKeys Technol, Stafford, VA USA. RP Holmberg, DG (reprint author), NIST, Mech Syst & Controls Grp, Div Energy & Environm, Engn Lab, Gaithersburg, MD 20899 USA. NR 13 TC 1 Z9 1 U1 0 U2 6 PU AMER SOC HEATING REFRIGERATING AIR-CONDITIONING ENG, INC, PI ATLANTA PA 1791 TULLIE CIRCLE NE, ATLANTA, GA 30329 USA SN 0001-2491 J9 ASHRAE J JI ASHRAE J. PD NOV PY 2012 VL 54 IS 11 BP B16 EP B19 PG 4 WC Thermodynamics; Construction & Building Technology; Engineering, Mechanical SC Thermodynamics; Construction & Building Technology; Engineering GA 039TE UT WOS:000311268600015 ER PT J AU Xie, SF Jin, MS Tao, J Wang, YC Xie, ZX Zhu, YM Xia, YN AF Xie, Shuifen Jin, Mingshang Tao, Jing Wang, Yucai Xie, Zhaoxiong Zhu, Yimei Xia, Younan TI Synthesis and Characterization of Pd@MxCu1-x (M=Au, Pd, and Pt) Nanocages with Porous Walls and a Yolk-Shell Structure through Galvanic Replacement Reactions SO CHEMISTRY-A EUROPEAN JOURNAL LA English DT Article DE copper; galvanic replacement; gold; nanocages; yolk-shell structure ID SHAPE-CONTROLLED SYNTHESIS; FACILE SYNTHESIS; METAL NANOSTRUCTURES; COPPER NANOCRYSTALS; OPTICAL-PROPERTIES; HOLLOW INTERIORS; CU2O NANOCAGES; GOLD NANOCAGES; ORGANIC MEDIUM; NANOPARTICLES AB This paper describes the synthesis of Pd@MxCu1-x (M=Au, Pd, and Pt) nanocages with a yolkshell structure through galvanic replacement reactions that involve Pd@Cu coreshell nanocubes as sacrificial templates and ethylene glycol as the solvent. Compared with the most commonly used templates based on Ag, Cu offers a much lower reduction potential (0.34 versus 0.80 V), making the galvanic reaction more easily to conduct, even at room temperature. Our structural and compositional characterizations indicated that the products were hollow inside, and each one of them contained porous MCu alloy walls and a Pd cube in the interior. For the Pd@AuxCu1-x yolkshell nanocages, they displayed broad extinction peaks extending from the visible to the near-IR region. Our mechanistic study revealed that the dissolution of the Cu shell preferred to start from the slightly truncated corners and then progressed toward the interior, because the Cu {100} side faces were protected by a surface capping layer of hexadecylamine. This galvanic approach can also be extended to generating other hollow metal nanostructures by using different combinations of Cu nanostructures and salt precursors. C1 [Xie, Shuifen; Wang, Yucai; Xia, Younan] Georgia Inst Technol, Wallace H Coulter Dept Biomed Engn, Atlanta, GA 30332 USA. [Xie, Shuifen; Wang, Yucai; Xia, Younan] Emory Univ, Sch Chem & Biochem, Atlanta, GA 30332 USA. [Xie, Shuifen; Wang, Yucai; Xia, Younan] Georgia Inst Technol, Sch Chem & Biomol Engn, Atlanta, GA 30332 USA. [Xie, Shuifen; Xie, Zhaoxiong] Xiamen Univ, Dept Chem, Coll Chem & Chem Engn, Xiamen 361005, Peoples R China. [Xie, Shuifen; Xie, Zhaoxiong] Xiamen Univ, State Key Lab Phys Chem Solid Surfaces, Xiamen 361005, Peoples R China. [Jin, Mingshang] Xi An Jiao Tong Univ, Frontier Inst Sci & Technol, Ctr Mat Chem, Xian 710049, Shaanxi, Peoples R China. [Tao, Jing; Zhu, Yimei] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RP Xia, YN (reprint author), Georgia Inst Technol, Wallace H Coulter Dept Biomed Engn, Atlanta, GA 30332 USA. EM younan.xia@bme.gatech.edu RI Xie, Zhaoxiong/G-3416-2010; Jin, Mingshang/F-4317-2011; SKL, PCOSS/D-4395-2013; wang, yucai/B-5388-2012; Xie, Shuifen/H-4484-2013; Xia, Younan/E-8499-2011; Wang, Yucai/A-1098-2017 OI Jin, Mingshang/0000-0001-9708-1959; wang, yucai/0000-0001-6046-2934; Xie, Shuifen/0000-0003-4283-6626; Wang, Yucai/0000-0001-6046-2934 FU NSF [DMR-1215034]; Georgia Institute of Technology; China Scholarship Council (CSC); U.S. Department of Energy, Basic Energy Sciences, by the Materials Sciences and Engineering Division [DE-AC02-98CH10886] FX This work was supported in part by a grant from the NSF (DMR-1215034) and start-up funds from Georgia Institute of Technology. As a visiting student from Xiamen University, S. X. was also partially supported by the China Scholarship Council (CSC). The work at BNL was supported by the U.S. Department of Energy, Basic Energy Sciences, by the Materials Sciences and Engineering Division under Contract No. DE-AC02-98CH10886 and through the use of CFN. NR 46 TC 25 Z9 26 U1 16 U2 232 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 0947-6539 J9 CHEM-EUR J JI Chem.-Eur. J. PD NOV PY 2012 VL 18 IS 47 BP 14974 EP 14980 DI 10.1002/chem.201202477 PG 7 WC Chemistry, Multidisciplinary SC Chemistry GA 037NC UT WOS:000311111900014 PM 23108763 ER PT J AU Wigington, BN Drummond, ML Cundari, TR Thorn, DL Hanson, SK Scott, SL AF Wigington, Bethany N. Drummond, Michael L. Cundari, Thomas R. Thorn, David L. Hanson, Susan K. Scott, Susannah L. TI A Biomimetic Pathway for Vanadium-Catalyzed Aerobic Oxidation of Alcohols: Evidence for a Base-Assisted Dehydrogenation Mechanism SO CHEMISTRY-A EUROPEAN JOURNAL LA English DT Article DE aerobic oxidation; base-assisted catalysis; biomimetic synthesis; Hammett correlation; vanadium ID ALPHA-HYDROXY ESTERS; GAUSSIAN-BASIS SETS; MOLECULAR-OXYGEN; SECONDARY ALCOHOLS; KINETIC RESOLUTION; QUINQUEVALENT VANADIUM; PROPARGYLIC ALCOHOLS; ORGANIC COMPOUNDS; MILD CONDITIONS; DECARBOXYLATION-DEOXYGENATION AB The first step in the catalytic oxidation of alcohols by molecular O2, mediated by homogeneous vanadium(V) complexes [LVV(O)(OR)], is ligand exchange. The unusual mechanism of the subsequent intramolecular oxidation of benzyl alcoholate ligands in the 8-hydroxyquinolinato (HQ) complexes [(HQ)2VV(O)(OCH2C6H4-p-X)] involves intermolecular deprotonation. In the presence of triethylamine, complex 3 (X=H) reacts within an hour at room temperature to generate, quantitatively, [(HQ)2VIV(O)], benzaldehyde (0.5 equivalents), and benzyl alcohol (0.5 equivalents). The base plays a key role in the reaction: in its absence, less than 12?% conversion was observed after 72 hours. The reaction is first order in both 3 and NEt3, with activation parameters ?H?=(28 +/- 4) kJ?mol-1 and ?S?=(-169 +/- 4) J?K-1?mol-1. A large kinetic isotope effect, 10.2 +/- 0.6, was observed when the benzylic hydrogen atoms were replaced by deuterium atoms. The effect of the para substituent of the benzyl alcoholate ligand on the reaction rate was investigated using a Hammett plot, which was constructed using sp. From the slope of the Hammett plot, ?=+(1.34 +/- 0.18), a significant buildup of negative charge on the benzylic carbon atom in the transition state is inferred. These experimental findings, in combination with computational studies, support an unusual bimolecular pathway for the intramolecular redox reaction, in which the rate-limiting step is deprotonation at the benzylic position. This mechanism, that is, base-assisted dehydrogenation (BAD), represents a biomimetic pathway for transition-metal-mediated alcohol oxidations, differing from the previously identified hydride-transfer and radical pathways. It suggests a new way to enhance the activity and selectivity of vanadium catalysts in a wide range of redox reactions, through control of the outer coordination sphere. C1 [Drummond, Michael L.; Cundari, Thomas R.] Univ N Texas, Dept Chem, Ctr Adv Sci Comp & Modeling CASCaM, Denton, TX 76201 USA. [Wigington, Bethany N.; Scott, Susannah L.] Univ Calif Santa Barbara, Dept Chem & Biochem, Santa Barbara, CA 93106 USA. [Thorn, David L.; Hanson, Susan K.] Los Alamos Natl Lab, Div Chem, Los Alamos, NM 87545 USA. [Scott, Susannah L.] Univ Calif Santa Barbara, Dept Chem Engn, Santa Barbara, CA 93106 USA. RP Cundari, TR (reprint author), Univ N Texas, Dept Chem, Ctr Adv Sci Comp & Modeling CASCaM, Denton, TX 76201 USA. EM thomas.cundari@unt.edu; skhanson@lanl.gov; sscott@engineering.ucsb.edu FU NSF through the Center for Enabling New Technologies through Catalysis (CENTC); ConvEne IGERT Program [NSF-DGE 0801627]; LANL Institute for Multiscale Materials Studies; MRSEC Program of the NSF [DMR 1121053]; NSF FX This work was supported by the NSF through the Center for Enabling New Technologies through Catalysis (CENTC). In addition, B.N.W acknowledges support from the ConvEne IGERT Program (NSF-DGE 0801627). S. K. H. thanks the LANL Institute for Multiscale Materials Studies for support. Portions of this work were performed using the Central Facilities of the Materials Research Laboratory at UC Santa Barbara, supported by the MRSEC Program of the NSF under Award No. DMR 1121053 and a member of the NSF-funded Materials Research Facilities Network (www.mrfn.org). NR 91 TC 21 Z9 22 U1 4 U2 106 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 0947-6539 J9 CHEM-EUR J JI Chem.-Eur. J. PD NOV PY 2012 VL 18 IS 47 BP 14981 EP 14988 DI 10.1002/chem.201202499 PG 8 WC Chemistry, Multidisciplinary SC Chemistry GA 037NC UT WOS:000311111900015 PM 23080554 ER PT J AU Park, SH Mei, CS Pauly, M Ong, RG Dale, BE Sabzikar, R Fotoh, H Nguyen, T Sticklen, M AF Park, Sang-Hyuck Mei, Chuansheng Pauly, Markus Ong, Rebecca Garlock Dale, Bruce E. Sabzikar, Robab Fotoh, Hussien Thang Nguyen Sticklen, Mariam TI Downregulation of Maize Cinnamoyl-Coenzyme A Reductase via RNA Interference Technology Causes Brown Midrib and Improves Ammonia Fiber Expansion-Pretreated Conversion into Fermentable Sugars for Biofuels SO CROP SCIENCE LA English DT Article ID ACID DETERGENT LIGNIN; COA REDUCTASE; ARABIDOPSIS-THALIANA; DIFFERENTIAL EXPRESSION; WALL DEGRADABILITY; KLASON LIGNIN; BIOSYNTHESIS; DIGESTIBILITY; LIGNIFICATION; GENES AB Conversion of lignocellulosic biomass into fermentable sugars for biofuels requires expensive pretreatment processes involving the breakdown of the cell wall structure and/or removal of lignin to increase accessibility of enzymes to the crop structural carbohydrates. Lignin is synthesized from precursors through a complex biosynthesis pathway. One of the important enzymes in this pathway is cinnamoyl-coenzyme A reductase (OCR), which catalyzes the transformation of feruloyl and p-coumaryl thioesters to their respective aldehydes. In an attempt to reduce lignin content and potentially accelerate deconstruction of maize (Zea mays L.) stover structural carbohydrates into fermentable sugars, expression of maize OCR (ZmCCR1; EC 1.2.1.44) was downregulated via ribonucleic acid interference (RNAi). Thirty first generation independent ZmCCR1_RNAi transgenic lines were produced. Among 10 out of 30 randomly tested, six lines showed significantly reduced ZmCCR1 transcription. The second generation of these ZmCCR1 downregulated transgenic plants exhibited brown coloration of midribs, husk, and stems and 7.0 to 8.7% reduction in Klason lignin. Also, crystalline cellulose was slightly increased in the lignin downregulated maize stover and further increased conversion of the ammonia fiber expansion (AFEX)-pretreated maize stover into fermentable sugars. The third generation of OCR downregulated plants showed further reduced OCR transcription as compared to their second generation of transgenic (T1) plants. C1 [Park, Sang-Hyuck; Sabzikar, Robab; Fotoh, Hussien; Thang Nguyen; Sticklen, Mariam] Michigan State Univ, Dep Crop & Soil Sci, E Lansing, MI 48824 USA. [Mei, Chuansheng] Inst Adv Learning & Res, Inst Sustainable & Renewable Resources, Danville, VA 24540 USA. [Pauly, Markus] Michigan State Univ, Dep Biochem & Mol Biol, E Lansing, MI 48824 USA. [Ong, Rebecca Garlock; Dale, Bruce E.] Michigan State Univ, Dep Chem Engn & Mat Sci, E Lansing, MI 48824 USA. [Ong, Rebecca Garlock; Dale, Bruce E.] Great Lakes Bioenergy Res Ctr, E Lansing, MI 48824 USA. RP Sticklen, M (reprint author), Michigan State Univ, Dep Crop & Soil Sci, E Lansing, MI 48824 USA. EM stickle1@msu.edu RI Pauly, Markus/B-5895-2008; OI Pauly, Markus/0000-0002-3116-2198; Ong, Rebecca/0000-0001-5020-646X FU Corn Marketing Program of Michigan (CMPM); Consortium for Plant Biotechnology Research (CPBR) FX The microscopic imaging was conducted via the services of the Michigan State University Center for Advanced Microscopy. Maize callus was obtained from the Maize Transformation Center of Iowa State University. The authors would like to thank Jeffrey R. Weatherhead of the MSU Plant Research Laboratory for his technical assistance on the carbohydrate analysis. This research was generously funded by the Corn Marketing Program of Michigan (CMPM) and the Consortium for Plant Biotechnology Research (CPBR). AFEX is a registered trademark of MBI International, Lansing, MI NR 70 TC 6 Z9 6 U1 0 U2 25 PU CROP SCIENCE SOC AMER PI MADISON PA 677 S SEGOE ROAD, MADISON, WI 53711 USA SN 0011-183X J9 CROP SCI JI Crop Sci. PD NOV-DEC PY 2012 VL 52 IS 6 BP 2687 EP 2701 DI 10.2135/cropsci2012.04.0253 PG 15 WC Agronomy SC Agriculture GA 028HP UT WOS:000310413700029 ER PT J AU Monazam, ER Breault, RW Siriwardane, R Tian, HJ Simonyi, T Carpenter, S AF Monazam, Esmail R. Breault, Ronald W. Siriwardane, Ranjani Tian, Hanjing Simonyi, Thomas Carpenter, Stephen TI Effect of Carbon Deposition on the Oxidation Rate of Copper/Bentonite in the Chemical Looping Process SO ENERGY & FUELS LA English DT Article; Proceedings Paper CT International Conference on Carbon Reduction Technologies CY SEP 19-22, 2011 CL Polish Jurrasic Highland, POLAND ID FIXED-BED REACTOR; OXYGEN CARRIERS; METAL-OXIDES; PHASE-CHANGE; COMBUSTION; KINETICS; METHANE; REDUCTION; PERFORMANCE AB The presented work is part of the Industrial Carbon Management Initiative (ICMI) on the development of metal oxide oxygen carriers, for use in the chemical looping combustion process. An oxygen carrier, CuO/bentonite. (60:40%), was reacted with methane gas and then oxidized in air. The change in weight and reaction gas concentrations Were measured using a thermogravimetric analyzer (TGA) equipped with a real time gas analyzer: The reduction-oxidation cycle was conducted within the temperature range of 750-900 degrees C for 10 cycles, using 20, 50, and 100% CH4 concentrationa in N-2 for the reduction segment and dry air for the oxidation segment Several analysis Methods were evaluated to fit the Oxidation of reduced CuO (Le., CO) data over the complete conversion range with suitable rate expression derived from existing. models for Oxidation, including the shrinking core model (diffusion and reaction control), first- and second order reaction rates, parallel and series reaction mechanisms, and Johnson-Mehl-Avrami (JMA) rate. The best agreement between the experimental data and the models of the Cu oxidation was accomplished using the JMA Model. The reactivity of the oxygen carrier during the oxidation reactions was affected by the CH4 concentration as well as the temperature. The rate of fractional uptake of oxygen onto the carrier decreased as the temperature increased, contrary to expectations and indicative that the mechanism is changing during the test. Analysis of the exit gas provided evidence of carbon deposition on the reduced sorbent particle and resulted in the CO2 product upon oxidation. The oxidation of this carbon releases significant heat that is capable of changing the particle morphology (Zhu, Y.; Mimura, K.; Isshiki, M. Oxid. Met 2004, 62, 207-222). On the basis of experimental results, the overall reaction process in the fuel reactor may be considered to consist of the decomposition of CH4 into C and H-2 and reduction of CuO/bentonite by the resulting H-2 and the parallel reaction of CH4 with CuO/bentonite. The extent of carbon deposition in the carrier particle increased with an increasing temperature and CH4 concentration. This deposited carbon not only leads to CO2 release from the oxidation reactor but, more importantly, causes degredation: of the carrier capacity and its reactivity. C1 [Monazam, Esmail R.; Breault, Ronald W.; Siriwardane, Ranjani; Tian, Hanjing; Simonyi, Thomas; Carpenter, Stephen] US DOE, Natl Energy Technol Lab, Morgantown, WV 26507 USA. [Monazam, Esmail R.] PLLC, REM Engn Serv, Morgantown, WV 26505 USA. [Tian, Hanjing; Simonyi, Thomas; Carpenter, Stephen] URS Energy & Construct Inc, Morgantown, WV 26505 USA. RP Breault, RW (reprint author), US DOE, Natl Energy Technol Lab, 3610 Collins Ferry Rd, Morgantown, WV 26507 USA. EM ronald.breault@netl.doe.gov OI Breault, Ronald/0000-0002-5552-4050 FU agency of the United States Government; Department of Energy through the Fossil Energy FX This report was prepared as an account of work sponsored by an agency of the United States Government. Neither the United States Government nor any agency thereof, nor any of their employees, makes any warranty, express or implied, or assumes any legal liability or responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would not infringe privately owned rights. Reference herein to any specific commercial product, process, or service by trade name, trademark, manufacturer, or otherwise does not necessarily constitute or imply its endorsement, recommendation, or favoring by the United States Government or any agency thereof. The views and opinions of authors expressed herein do not necessarily state or reflect those of the United States Government or any agency thereof.; The authors acknowledge the Department of Energy for funding the research through the Fossil Energy's Gasification Technology and Advanced Research funding programs. NR 19 TC 4 Z9 4 U1 3 U2 32 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0887-0624 EI 1520-5029 J9 ENERG FUEL JI Energy Fuels PD NOV PY 2012 VL 26 IS 11 BP 6576 EP 6583 DI 10.1021/ef301389h PG 8 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA 039KO UT WOS:000311244900015 ER PT J AU Heufer, KA Sarathy, SM Curran, HJ Davis, AC Westbrook, CK Pitz, WJ AF Heufer, K. Alexander Sarathy, S. Mani Curran, Henry J. Davis, Alexander C. Westbrook, Charles K. Pitz, William J. TI Detailed Kinetic Modeling Study of n-Pentanol Oxidation SO ENERGY & FUELS LA English DT Article; Proceedings Paper CT International Conference on Carbon Reduction Technologies CY SEP 19-22, 2011 CL Polish Jurrasic Highland, POLAND ID HIGHER-ALCOHOL/GASOLINE BLENDS; HIGH-TEMPERATURE OXIDATION; RAPID COMPRESSION MACHINE; SHOCK-TUBE; PREMIXED FLAMES; ETHANOL OXIDATION; METHYL BUTANOATE; COMBUSTION; IGNITION; CHEMISTRY AB To help overcome the world's dependence upon fossil fuels, suitable biofuels are promising alternatives that can be used in the transportation sector. Recent research on internal combustion engines shows that short alcoholic fuels (e.g., ethanol or n-butanol) have reduced pollutant emissions and increased knock resistance,compared to fossil fuels. Although higher molecular weight alcohols (e.g., n-pentanol and n-hexanol) exhibit higher reactivity that lowers their knock resistance, they are suitable for diesel engines or advanced engine concepts, such as homogeneous charge compression ignition (HCCI), where higher reactivity at lower temperatures is necessary for engine operation The present study presents a detailed kinetic model for n-pentanol based on modeling rules previously presented for n-butanol. This approach was initially validated using quantum chemistry calculations to verify the most stable n-pentanol conformation and to obtain C-H and C-C bond dissociation energies: The proposed model has been validated against ignition delay time data, speciation data from a Jet stirred reactor, and laminar flame velocity measurements. Overall, the model shows good agreement with the experiments and permits a detailed discussion of the differences between alcohols and alkanes. C1 [Heufer, K. Alexander; Curran, Henry J.] Natl Univ Ireland Galway, Galway, Ireland. [Sarathy, S. Mani; Davis, Alexander C.] King Abdullah Univ Sci & Technol, Clean Combust Res Ctr, Thuwal 239556900, Saudi Arabia. [Westbrook, Charles K.; Pitz, William J.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Heufer, KA (reprint author), Natl Univ Ireland Galway, Univ Rd, Galway, Ireland. EM alexander.heufer@nuigalway.ie RI Davis, Alexander/F-3153-2013; Heufer, Karl Alexander/O-3892-2014; Sarathy, S. Mani/M-5639-2015; OI Sarathy, S. Mani/0000-0002-3975-6206; Curran, Henry/0000-0002-5124-8562 FU U.S. Department of Energy [DE-AC52-07NA27344]; King Abdullah University of Science and Technology FX The work performed at the Clean Combustion Research Center acknowledges research funding from the King Abdullah University of Science and Technology. The work performed at LLNL was performed under the auspices of the U.S. Department of Energy under Contract DE-AC52-07NA27344. NR 52 TC 37 Z9 38 U1 9 U2 79 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0887-0624 EI 1520-5029 J9 ENERG FUEL JI Energy Fuels PD NOV PY 2012 VL 26 IS 11 BP 6678 EP 6685 DI 10.1021/ef3012596 PG 8 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA 039KO UT WOS:000311244900026 ER PT J AU Harendra, S Oryshcyhn, D Gerdemann, S Ochs, T Clark, J AF Harendra, Sivaram Oryshcyhn, Danylo Gerdemann, Stephen Ochs, Thomas Clark, John TI Modeling Energy Flow in an Integrated Pollutant Removal (IPR) System with CO2 Capture Integrated with Oxy-fuel Combustion SO ENERGY & FUELS LA English DT Article; Proceedings Paper CT International Conference on Carbon Reduction Technologies CY SEP 19-22, 2011 CL Polish Jurrasic Highland, POLAND ID FLUE-GAS; IGCC; OPTIMIZATION; SIMULATION; RECOVERY AB Oxy-coal combustion is one of the technical solutions for Mitigating CO2 in thermal power plants. :Many processes have been evolved in past the decade to capture CO2 from processes industries, Researchers at the National Energy Technology Laboratory (NETL) have patented a process, integrated pollutant removal (IPR), that uses off the shelf technology to produce a sequestration-ready CO2 stream from an oxy-combustion power plant. The IPR process as it is realized at the Jupiter Oxygen Burner Test Facility is a spray tower (direct-contact heat exchanger) followed by four stages of compression with intercooling. To study the energy flows of the oxy-combustion process, a 15 MWth oxy-combustion pulverized-coal-fired plant integrated-With the IPR system was simulated and analyzed using ASPEN Plus and ASPEN energy analyzer. This paper discusses flue-gas recycle, energy flow, recovery, and optimization of IPR systems. ASPEN models of heat.: and mass-transfer processes in a flue-gas-condensing heat-exchanger system were developed to predict the :heat transferred from flue gas to cooling water. The flue-gas. exit temperature, cooling water outlet temperature, and energy flows of IPR streams Were computed using ASPEN model's. Pinch principles are deployed for targeting design and operation-guiding purposes and balancing the heat and mass transfer in the IPR system. The results are expected to support sophistication of the IPR system design, improving its application in a variety of settings. They open the door for valuable IPR efficiency improvements and generalization of methodology for simultaneous Management of energy resources. C1 [Harendra, Sivaram; Oryshcyhn, Danylo; Gerdemann, Stephen; Ochs, Thomas; Clark, John] US DOE, Proc Dev Div, NETL, Albany, OR 97321 USA. RP Harendra, S (reprint author), US DOE, Proc Dev Div, NETL, Albany, OR 97321 USA. EM harendrs@netl.doe.gov FU Oak Ridge Institute for Science and Education (ORISE) at the National Energy Technology Laboratory (NETL); Department of Energy (DOE) FX This study was supported by the Oak Ridge Institute for Science and Education (ORISE) at the National Energy Technology Laboratory (NETL) with funding from the Department of Energy (DOE). NR 15 TC 1 Z9 1 U1 1 U2 30 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0887-0624 EI 1520-5029 J9 ENERG FUEL JI Energy Fuels PD NOV PY 2012 VL 26 IS 11 BP 6930 EP 6937 DI 10.1021/ef301500g PG 8 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA 039KO UT WOS:000311244900053 ER PT J AU Peters, VA Manley, DK AF Peters, Valerie A. Manley, Dawn K. TI An examination of fuel consumption trends in construction projects SO ENERGY POLICY LA English DT Article DE Construction equipment; Fuel consumption; Fuel economy ID EMISSIONS AB Recent estimates of fuel consumption in construction projects are highly variable. Lack of standards for reporting at both the equipment and project levels make it difficult to quantify the magnitude of fuel consumption and the associated opportunities for efficiency improvements in construction projects. In this study, we examined clusters of Environmental Impact Reports for seemingly similar construction projects in California. We observed that construction projects are not characterized consistently by task or equipment. We found wide variations in estimates for fuel use in terms of tasks, equipment, and overall projects, which may be attributed in part to inconsistencies in methodology and parameter ranges. Our analysis suggests that standardizing fuel consumption reporting and estimation methodologies for construction projects would enable quantification of opportunities for efficiency improvements at both the equipment and project levels. With increasing emphasis on reducing fossil fuel consumption, it will be important to quantify opportunities to increase fuel efficiency, including across the construction sector. (C) 2012 Elsevier Ltd. All rights reserved. C1 [Peters, Valerie A.; Manley, Dawn K.] Sandia Natl Labs, Livermore, CA 94550 USA. RP Manley, DK (reprint author), Sandia Natl Labs, 7011 East Ave, Livermore, CA 94550 USA. EM vapeter@sandia.gov; dmanley@sandia.gov FU Laboratory Directed Research and Development program at Sandia National Laboratories; U S Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was funded by the Laboratory Directed Research and Development program at Sandia National Laboratories. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U S Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL85000. NR 45 TC 2 Z9 2 U1 0 U2 4 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0301-4215 J9 ENERG POLICY JI Energy Policy PD NOV PY 2012 VL 50 BP 496 EP 506 DI 10.1016/j.enpol.2012.07.048 PG 11 WC Energy & Fuels; Environmental Sciences; Environmental Studies SC Energy & Fuels; Environmental Sciences & Ecology GA 028EO UT WOS:000310405800047 ER PT J AU Ke, J Price, L Ohshita, S Fridley, D Khanna, NZ Zhou, N Levine, M AF Ke, Jing Price, Lynn Ohshita, Stephanie Fridley, David Khanna, Nina Zheng Zhou, Nan Levine, Mark TI China's industrial energy consumption trends and impacts of the Top-1000 Enterprises Energy-Saving Program and the Ten Key Energy-Saving Projects SO ENERGY POLICY LA English DT Article DE Industry; Energy intensity; Decomposition ID INDEX DECOMPOSITION APPROACH; RELATIVE IMPORTANCE; INTENSITY CHANGE AB This study analyzes China's industrial energy consumption trends from 1996 to 2010 with a focus on the impact of the Top-1000 Enterprises Energy-Saving Program and the Ten Key Energy-Saving Projects. From 1996 to 2010, China's industrial energy consumption increased by 134%, even as the industrial economic energy intensity decreased by 46%. Decomposition analysis shows that the production effect was the dominant cause of the rapid growth in industrial energy consumption, while the efficiency effect was the major factor slowing the growth of industrial energy consumption. The structural effect had a relatively small and fluctuating influence. Analysis shows the strong association of industrial energy consumption with the growth of China's economy and changing energy policies. An assessment of the Top-1000 Enterprises Energy-Saving Program and the Ten Key Energy-Saving Projects indicates that the economic energy intensity of major energy-intensive industrial sub-sectors, as well as the physical energy intensity of major energy-intensive industrial products, decreased significantly during China's 11th Five Year Plan (FYP) period (2006-2010). This study also shows the importance and challenge of realizing structural change toward less energy-intensive activities in China during the 12th FYP period (2011-2015). (C) 2012 Elsevier Ltd. All rights reserved. C1 [Ke, Jing; Price, Lynn; Ohshita, Stephanie; Fridley, David; Khanna, Nina Zheng; Zhou, Nan; Levine, Mark] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Energy Anal & Environm Impacts Dept, Berkeley, CA 94720 USA. [Ohshita, Stephanie] Univ San Francisco, Dept Environm Sci, Coll Arts & Sci, San Francisco, CA 94117 USA. RP Ke, J (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Energy Anal & Environm Impacts Dept, 1 Cyclotron Rd,MS 90R4000, Berkeley, CA 94720 USA. EM jke@lbl.gov RI Ke, Jing/H-4816-2016 OI Ke, Jing/0000-0002-5972-8042 FU Energy Foundation; Dow Chemical Company through Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Energy Foundation and Dow Chemical Company (through a charitable contribution) through the Department of Energy under Contract no. DE-AC02-05CH11231. The authors thank the anonymous reviewers for their valuable comments and suggestions. NR 48 TC 25 Z9 27 U1 1 U2 24 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0301-4215 J9 ENERG POLICY JI Energy Policy PD NOV PY 2012 VL 50 BP 562 EP 569 DI 10.1016/j.enpol.2012.07.057 PG 8 WC Energy & Fuels; Environmental Sciences; Environmental Studies SC Energy & Fuels; Environmental Sciences & Ecology GA 028EO UT WOS:000310405800053 ER PT J AU Larsen, PH Goldman, CA Satchwell, A AF Larsen, Peter H. Goldman, Charles A. Satchwell, Andrew TI Evolution of the U.S. energy service company industry: Market size and project performance from 1990-2008 SO ENERGY POLICY LA English DT Article DE ESCO; Energy services industry size; Project performance ID ESCO INDUSTRY AB The U.S. energy service company (ESCO) industry is an example of a private sector business model where energy savings are delivered to customers primarily through the use of performance-based contracts. This study was conceived as a snapshot of the ESCO industry prior to the economic slowdown and the introduction of federal stimulus funding mandated by enactment of the American Recovery and Reinvestment Act of 2009 (ARRA). This study utilizes two parallel analytic approaches to characterize ESCO industry and market trends in the U.S.: (1) a "top-down" approach involving a survey of individual ESCOs to estimate aggregate industry activity and (2) a "bottom-up" analysis of a database of similar to 3250 projects (representing over $8B in project investment) that reports market trends including installed EE retrofit strategies, project installation costs and savings, project payback times, and benefit-cost ratios over time. Despite the onset of a severe economic recession, the U.S. ESCO industry managed to grow at about 7% per year between 2006 and 2008. ESCO industry revenues were about $4.1 billion in 2008 and ESCOs anticipate accelerated growth through 2011 (25% per year). We found that 2484 ESCO projects in our database generated similar to$4.0 billion ($2009) in net, direct economic benefits to their customers. We estimate that the ESCO project database includes about 20% of all U.S. ESCO market activity from 1990-2008. Assuming the net benefits per project are comparable for ESCO projects that are not included in the LBNL database, this would suggest that the ESCO industry has generated similar to$23 billion in net direct economic benefits for customers at projects installed between 1990 and 2008. There is empirical evidence confirming that the industry is evolving by installing more comprehensive and complex measures-including onsite generation and measures to address deferred maintenance-but this evolution has significant implications for customer project economics, especially at K-12 schools. We found that the median simple payback time has increased from 1.9 to 3.2 years in private sector projects since the early-to-mid 1990s and from 5.2 to 10.5 years in public sector projects for the same time period. (C) 2012 Elsevier Ltd. All rights reserved. C1 [Larsen, Peter H.; Goldman, Charles A.; Satchwell, Andrew] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Energy Anal & Environm Impacts Dept, Berkeley, CA 94720 USA. [Larsen, Peter H.] Stanford Univ, Management Sci & Engn Dept, Sch Engn, Stanford, CA 94305 USA. RP Larsen, PH (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Energy Anal & Environm Impacts Dept, 1 Cyclotron Rd,MS 90-4000, Berkeley, CA 94720 USA. EM PHLarsen@lbl.gov FU Department of Energy's Office of Energy Efficiency and Renewable Energy (EERE); Weatherization and Intergovernmental Program [DE-AC02-05CH11231] FX The work described in this report was funded by the Department of Energy's Office of Energy Efficiency and Renewable Energy (EERE), Weatherization and Intergovernmental Program under Contract no. DE-AC02-05CH11231. The authors would like to thank Anna Garcia, Timothy Unruh, Roya Stanley, Chani Vines, and Chip Goyette (DOE Office of Energy Efficiency and Renewable Energy) for supporting this project; Donald Gilligan, Terry E. Singer (NAESCO), David Birr (Synchronous Energy Solutions), and Patricia Donahue for technical advice; and Steve Schiller (Schiller Consulting) and David Belzer (Pacific Northwest National Laboratory) for providing comments on earlier drafts of this research. The authors would like to thank Ranjit Bharvikar and Elizabeth Stuart for their assistance during various stages of this project. John Shonder of Oak Ridge National Laboratory provided valuable information on FEMP ESPC contracts. The authors also gratefully acknowledge Nicole Hopper for her suggestions on the initial scope of this analysis as well as her significant research into the early evolution of this industry. Finally, we thank three anonymous reviewers for helpful suggestions. All remaining errors and omissions are the responsibility of the authors. NR 42 TC 18 Z9 19 U1 2 U2 35 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0301-4215 J9 ENERG POLICY JI Energy Policy PD NOV PY 2012 VL 50 BP 802 EP 820 DI 10.1016/j.enpol.2012.08.035 PG 19 WC Energy & Fuels; Environmental Sciences; Environmental Studies SC Energy & Fuels; Environmental Sciences & Ecology GA 028EO UT WOS:000310405800074 ER PT J AU Post, ES Grambsch, A Weaver, C Morefield, P Huang, J Leung, LY Nolte, CG Adams, P Liang, XZ Zhu, JH Mahoney, H AF Post, Ellen S. Grambsch, Anne Weaver, Chris Morefield, Philip Huang, Jin Leung, Lai-Yung Nolte, Christopher G. Adams, Peter Liang, Xin-Zhong Zhu, Jin-Hong Mahoney, Hardee TI Variation in Estimated Ozone-Related Health Impacts of Climate Change due to Modeling Choices and Assumptions SO ENVIRONMENTAL HEALTH PERSPECTIVES LA English DT Article DE climate change; mortality; ozone; population projections; sensitivity analysis ID MORTALITY AB BACKGROUND: Future climate change may cause air quality degradation via climate-induced changes in meteorology, atmospheric chemistry, and emissions into the air. Few studies have explicitly modeled the potential relationships between climate change, air quality, and human health, and fewer still have investigated the sensitivity of estimates to the underlying modeling choices. OBJECTIVES: Our goal was to assess the sensitivity of estimated ozone-related human health impacts of climate change to key modeling choices. METHODS: Our analysis included seven modeling systems in which a climate change model is linked to an air quality model, five population projections, and multiple concentration response functions. Using the U.S. Environmental Protection Agency's (EPA's) Environmental Benefits Mapping and Analysis Program (BenMAP), we estimated future ozone (O-3)-related health effects in the United States attributable to simulated climate change between the years 2000 and approximately 2050, given each combination of modeling choices. Health effects and concentration response functions were chosen to match those used in the U.S. EPA's 2008 Regulatory Impact Analysis of the National Ambient Air Quality Standards for O-3. RESULTS: Different combinations of methodological choices produced a range of estimates of national O-3-related mortality from roughly 600 deaths avoided as a result of climate change to 2,500 deaths attributable to climate change (although the large majority produced increases in mortality). The choice of the climate change and the air quality model reflected the greatest source of uncertainty, with the other modeling choices having lesser but still substantial effects. CONCLUSIONS: Our results highlight the need to use an ensemble approach, instead of relying on any one set of modeling choices, to assess the potential risks associated with O-3-related human health effects resulting from climate change. C1 [Post, Ellen S.; Huang, Jin; Mahoney, Hardee] ABT Associates Inc, Environm & Resources Div, Bethesda, MD 20814 USA. [Grambsch, Anne; Weaver, Chris; Morefield, Philip] US EPA, Off Res & Dev, Global Change Res Program, Natl Ctr Environm Assessment, Washington, DC 20460 USA. [Leung, Lai-Yung] Pacific NW Natl Lab, Richland, WA USA. [Nolte, Christopher G.] US EPA, Natl Exposure Res Lab, Athens, GA USA. [Adams, Peter] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Liang, Xin-Zhong; Zhu, Jin-Hong] Univ Illinois, Dept Atmospher Sci, Urbana, IL 61801 USA. RP Huang, J (reprint author), ABT Associates Inc, Environm & Resources Div, 4550 Montgomery Ave,Suite 800, Bethesda, MD 20814 USA. EM jin_huang@abtassoc.com RI Nolte, Christopher/H-4345-2012; Weaver, Christopher/G-3714-2010; Adams, Peter/D-7134-2013 OI Nolte, Christopher/0000-0001-5224-9965; Weaver, Christopher/0000-0003-4016-5451; Adams, Peter/0000-0003-0041-058X FU U.S. Environmental Protection Agency (EPA) [RD-83337301-0]; Abt Associates Inc.; U.S. EPA [EP-D-08-100] FX Support for this analysis was funded through the U.S. Environmental Protection Agency (EPA) award RD-83337301-0. Additional support, provided by Abt Associates Inc., was funded through U.S. EPA Contract EP-D-08-100. The views expressed in this document are solely those of the authors and do not represent official U.S. EPA policy. NR 28 TC 24 Z9 24 U1 1 U2 38 PU US DEPT HEALTH HUMAN SCIENCES PUBLIC HEALTH SCIENCE PI RES TRIANGLE PK PA NATL INST HEALTH, NATL INST ENVIRONMENTAL HEALTH SCIENCES, PO BOX 12233, RES TRIANGLE PK, NC 27709-2233 USA SN 0091-6765 J9 ENVIRON HEALTH PERSP JI Environ. Health Perspect. PD NOV PY 2012 VL 120 IS 11 BP 1559 EP 1564 DI 10.1289/ehp.1104271 PG 6 WC Environmental Sciences; Public, Environmental & Occupational Health; Toxicology SC Environmental Sciences & Ecology; Public, Environmental & Occupational Health; Toxicology GA 036ZE UT WOS:000311070000025 PM 22796531 ER PT J AU Zhu, JX Bishop, AR AF Zhu, Jian-Xin Bishop, A. R. TI Quasiparticle scattering interference in (K, Tl)FexSe2 superconductors SO EPL LA English DT Article ID STATES; INSULATOR AB We model the quasiparticle interference (QPI) pattern in the recently discovered (K, Tl)FexSe2 superconductors. We show in the superconducting state that, due to the absence of hole pockets at the Brillouin zone center, the quasiparticle scattering occurs around the momentum transfer q=(0, 0) and (+/-pi, +/-pi) between electron pockets located at the zone boundary. More importantly, although both d(x2-y2)-wave and s-wave pairing symmetry lead to nodeless quasiparticle excitations, distinct QPI features are predicted between both types of pairing symmetry. The so-called Z-map of the QPI exhibits strongest scattering with q = (+/-pi, +/-pi) for the d(x2-y2)-wave pairing symmetry, which is absent in the case of an isotropic s-wave pairing symmetry. The significant contrast in the QPI pattern between the d(x2-y2)-wave and the isotropic s-wave pairing symmetry can be used to probe the pairing symmetry within the Fourier-transform STM technique. Copyright (C) EPLA, 2012 C1 [Zhu, Jian-Xin] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Bishop, A. R.] Los Alamos Natl Lab, PADSTE, Los Alamos, NM 87545 USA. RP Zhu, JX (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. OI Zhu, Jianxin/0000-0001-7991-3918 FU U.S. DOE at LANL [DE-AC52-06NA25396]; U.S. DOE Office of Basic Energy Sciences FX One of us (J-XZ) acknowledges useful discussions with A. V. BALATSKY. This work was supported by U.S. DOE at LANL under Contract No. DE-AC52-06NA25396 and the U.S. DOE Office of Basic Energy Sciences. NR 39 TC 3 Z9 3 U1 4 U2 15 PU EPL ASSOCIATION, EUROPEAN PHYSICAL SOCIETY PI MULHOUSE PA 6 RUE DES FRERES LUMIERE, MULHOUSE, 68200, FRANCE SN 0295-5075 J9 EPL-EUROPHYS LETT JI EPL PD NOV PY 2012 VL 100 IS 3 AR 37004 DI 10.1209/0295-5075/100/37004 PG 6 WC Physics, Multidisciplinary SC Physics GA 042RD UT WOS:000311487800029 ER PT J AU Stanley, FE AF Stanley, F. E. TI A beginner's guide to uranium chronometry in nuclear forensics and safeguards SO JOURNAL OF ANALYTICAL ATOMIC SPECTROMETRY LA English DT Review ID ACCELERATOR MASS-SPECTROMETRY; HIGHLY ENRICHED URANIUM; OPEN SYSTEM MODEL; ICP-MS; AGE; METHODOLOGY AB Nuclear forensics and international safeguards are rising in importance in the face of increasing concerns over the illicit production and trafficking of nuclear materials worldwide. One of the most valuable approaches in such efforts is the chronometric investigation ("age-dating") of collected/interdicted materials; well-designed chronometric schemes may simultaneously provide insight into a sample's composition, enrichment history, and the time elapsed since last purification. Given the importance of this analytical approach in obtaining valuable material signatures, a thorough understanding of age-dating principles and special concerns will be of significant value to the rising generation of scientists interrogating nuclear materials collected around the world. In this work, the fundamental concepts of uranium chronometry are discussed, along with several unique concerns and recent applications associated with the use of age-dating approaches in this manner. As significant work remains to be done in these fields, several potential concepts for future development are also highlighted. C1 Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Stanley, FE (reprint author), Los Alamos Natl Lab, TA 3,Bldg 29,Diamond Dr, Los Alamos, NM 87545 USA. EM floyd@lanl.gov NR 39 TC 12 Z9 12 U1 0 U2 52 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 0267-9477 J9 J ANAL ATOM SPECTROM JI J. Anal. At. Spectrom. PD NOV PY 2012 VL 27 IS 11 BP 1821 EP 1830 DI 10.1039/c2ja30182b PG 10 WC Chemistry, Analytical; Spectroscopy SC Chemistry; Spectroscopy GA 029FJ UT WOS:000310479900001 ER PT J AU Nigra, MM Arslan, I Katz, A AF Nigra, Michael M. Arslan, Ilke Katz, Alexander TI Gold nanoparticle-catalyzed reduction in a model system: Quantitative determination of reactive heterogeneity of a supported nanoparticle surface SO JOURNAL OF CATALYSIS LA English DT Article DE Gold nanoparticle; Catalysis; Corner; Edge; Coordinative unsaturation; Resazurin; Electron transfer ID SELF-ASSEMBLED MONOLAYERS; GAS SHIFT CATALYSIS; AU(111); SIZE; SITES; TEMPERATURE; SELECTIVITY; ADSORPTION; DEPOSITION; OXIDATION AB Kinetic poisoning experiments employing organic ligands were conducted using a gold nanoparticle-catalyzed reaction consisting of the reduction of resazurin to resorufin. The kinetic contributions of three distinct types of sites along with the number density of each of these site types during reaction were determined. The calculated number densities of each of the three types of sites, hypothesized to be corners, edges, and terraces, correlates well with atomic-resolution micrographs of the supported gold nanoparticles, obtained using aberration-corrected transmission electron microscopy and with predictions based on geometric models of idealized gold nanoparticles. The most active sites comprising 1% of the surface atoms exhibit at least 30% of the total activity of the catalyst for resazurin reduction. The selective mechanical blocking of surface sites on nanoparticles, particularly undercoordinated sites, paves the way for novel approaches utilizing organic ligands to quantify the activity of different active sites and control catalysis on metal surfaces. (C) 2012 Elsevier Inc. All rights reserved. C1 [Nigra, Michael M.; Katz, Alexander] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Arslan, Ilke] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Katz, A (reprint author), Univ Calif Berkeley, Dept Chem & Biomol Engn, 201 Gilman Hall, Berkeley, CA 94720 USA. EM askatz@berkeley.edu RI Foundry, Molecular/G-9968-2014 FU Chevron Corporation; National Science Foundation [CBET 0854560]; U.S. Department of Energy [DE-SC0005822, DE-AC02-05CH11231]; National Center for Electron Microscopy, Lawrence Berkeley Lab; Laboratory Directed Research and Development program at the Pacific Northwest National Laboratory (PNNL); BER; U.S. DOE [DE-AC05-76RL01830] FX The authors acknowledge helpful discussions with Prof. Yaron Paz at Technion in Haifa, Israel, and Prof. Matthew Neurock at University of Virginia. We are grateful to the Management and Transfer of Hydrogen via Catalysis Program funded by Chevron Corporation, the National Science Foundation (CBET 0854560), and U.S. Department of Energy under contract DE-SC0005822 for financial support. The authors acknowledge support of the National Center for Electron Microscopy, Lawrence Berkeley Lab, which is supported by the U.S. Department of Energy under contract DE-AC02-05CH11231. This work was supported in part by the Laboratory Directed Research and Development program at the Pacific Northwest National Laboratory (PNNL). The aberration-corrected electron microscopy was performed in the William R. Wiley Environmental Molecular Sciences Laboratory, a U.S. Department of Energy (DOE) national scientific user facility located at PNNL and funded by BER. PNNL is operated by Battelle for the U.S. DOE under contract DE-AC05-76RL01830. NR 42 TC 11 Z9 11 U1 4 U2 69 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9517 J9 J CATAL JI J. Catal. PD NOV PY 2012 VL 295 BP 115 EP 121 DI 10.1016/j.jcat.2012.08.001 PG 7 WC Chemistry, Physical; Engineering, Chemical SC Chemistry; Engineering GA 035IP UT WOS:000310940300011 ER PT J AU Ciftlikli, EZ Lallo, J Lee, EYM Rangan, S Senanayake, SD Hinch, BJ AF Ciftlikli, E. Z. Lallo, J. Lee, E. Y. -M. Rangan, S. Senanayake, S. D. Hinch, B. J. TI Competing pathways for isocyanate loss from Cu(001) with co-adsorbed oxygen SO JOURNAL OF CATALYSIS LA English DT Article DE Isocyanate; Cyanide; Oxidation; Dissociation; Copper; Surfaces ID NOBLE-METAL CATALYSTS; ELECTRON-ENERGY LOSS; SURFACE-CHEMISTRY; TDS MEASUREMENTS; NITROGEN-OXIDE; MFI ZEOLITE; NO; CO; REDUCTION; ADSORPTION AB Cu(001)-bound isocyanate species (Nco((a))) have been prepared with two distinct methods. Isocyanic acid (HNCO) exposures at room temperature resulted in adsorbed NCO(a) alone. The exposure of Cu(001) to cyanogen (C2N2) and O-2 leads to surfaces displaying co-adsorbed oxygen (O-(a)), cyanide (CN(a)), and NCO(a) species. O-2 exposure of submonolayer NCO/Cu(001), followed by brief annealing at 473 K, initiated NCO(a) oxidation, giving rise to CO2(g) desorption and a surface-bound atomic N-(a) species. CO2(g) evolution was observed over a wide range of initial O-(a) coverages. In contrast, comparable thermal treatments of CN + O + NCO/Cu(001) samples, at 473 K, yield both CO(g) and CO2(g). Both TPRD and XPS studies of pre- and post-annealed surfaces indicated the two gaseous products. The co-adsorption of CN(a) promotes the dissociation of NCO(a) into CO(g) and N-(a), and dissociation can become the dominant means for NCO(a) removal. (C) 2012 Elsevier Inc. All rights reserved. C1 [Ciftlikli, E. Z.; Lallo, J.; Lee, E. Y. -M.; Rangan, S.; Hinch, B. J.] Rutgers State Univ, Dept Chem & Chem Biol, Piscataway, NJ 08854 USA. [Senanayake, S. D.] Oak Ridge Natl Lab, Oak Ridge, TN 37830 USA. RP Hinch, BJ (reprint author), Rutgers State Univ, Dept Chem & Chem Biol, 610 Taylor Rd, Piscataway, NJ 08854 USA. EM jhinch@rutchem.rutgers.edu RI Rangan, Sylvie/H-6522-2013; Senanayake, Sanjaya/D-4769-2009 OI Senanayake, Sanjaya/0000-0003-3991-4232 FU NSF [CHE-0718055, CHE-1124879]; Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy [DE-AC05-00OR22725]; Oak Ridge National Laboratory; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX The work was funded by the NSF award CHE-0718055 and in part by CHE-1124879. The U12a beamline was supported by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy, under contract DE-AC05-00OR22725 with Oak Ridge National Laboratory. SDS was funded through the ORNL directly. The National Synchrotron Light Source, Brookhaven National Laboratory, was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. NR 48 TC 0 Z9 0 U1 3 U2 27 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9517 EI 1090-2694 J9 J CATAL JI J. Catal. PD NOV PY 2012 VL 295 BP 269 EP 273 DI 10.1016/j.jcat.2012.08.009 PG 5 WC Chemistry, Physical; Engineering, Chemical SC Chemistry; Engineering GA 035IP UT WOS:000310940300027 ER PT J AU Haranczyk, M Urbaszek, P Ng, EG Puzyn, T AF Haranczyk, Maciej Urbaszek, Piotr Ng, Esmond G. Puzyn, Tomasz TI Combinatorial x Computational x Cheminformatics (C-3) Approach to Characterization of Congeneric Libraries of Organic Pollutants SO JOURNAL OF CHEMICAL INFORMATION AND MODELING LA English DT Article ID DESCRIPTORS; TAUTOMERS; DIOXINS; QSPR AB Congeners are molecules based on the same carbon skeleton but are different by the number of substituents and/or a substitution pattern. Examples are 1-chloronaphthalene, 1,4-dichloronaplithalene, and 1,3,8-trichloronaphthalene. Various persistent :Organic pollutants (POPs) exist in the environment as families; of congeners. Very large numbers of possible; congeners Make their experimental characterization and risk assessment unfeasible. Computational high throughput and quantitative structure property relationship, (QSPR) modeling. has been :limited by the lack of tools and approaches facilitating analysis of such POP families. We present a comprehensive :approach that enables modeling of extremely large congeneric libraries. The approach involves three steps: (1) combinatorial generation of a library of congeners, (2) quantum chemical characterization of each structure at the PM6 seiniempirical level to obtain molecular descriptors, and (3) analysis of the information generated in step 2 In steps 1-3, we employ combinatorial, computational, and cheminformatics techniques,, respectively. Therefore,,this hybrid approach is named Combinatorial :X Computational x Cheminformatics", or just abbreviated as C-3 (or C:cubed) approach. We demonstrate the usefulness of this approach by generating and characterizing Br- and Cl- substituted congeneric families of 23 typical POPs. The analysis of the resulting Set Of 1 840 95,1 congeners that includes Cl-, Br-,. and mixed Br/Cl-substituted species, proves that, based on structural similarities defined by the molecular descriptors values, the existing QSPR models developed originally for Cl-. and Br-substitufed Corigeners can be applied also to mixed Br/Cl-substituted Thus, the C-3-aPProach,May serve is a tool for exploring structural applicability domains of the existing QSPRmodels for congeneric sets. C1 [Haranczyk, Maciej; Ng, Esmond G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, Berkeley, CA 94720 USA. [Urbaszek, Piotr; Puzyn, Tomasz] Univ Gdansk, Dept Chem, Lab Environm Chemometr, PL-80952 Gdansk, Poland. RP Haranczyk, M (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, 1 Cyclotron Rd,Mail Stop 50E-1650, Berkeley, CA 94720 USA. EM mharanczyk@lbl.gov RI Haranczyk, Maciej/A-6380-2014 OI Haranczyk, Maciej/0000-0001-7146-9568 FU U.S. Department of Energy [DE-AC02-05CH11231]; Polish Ministry of Science and Higher Education [DS/530-8180-D202-12]; Foundation for Polish Science [FOCUS 559-8430.1251-0]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX We would like to thank Dr. James Stewart for providing a MOPAC software license. We acknowledge the fruitful discussions with Noriyuld Suzuki. This research was supported in part (to M.H. and E.G.N.) by the U.S. Department of Energy under contract DE-AC02-05CH11231. This work was supported (to P.U. and T.P.) by the Polish Ministry of Science and Higher Education (Grant No. DS/530-8180-D202-12) and the Foundation for Polish Science (Grant No. FOCUS 559-8430.1251-0). This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 32 TC 5 Z9 5 U1 0 U2 12 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1549-9596 J9 J CHEM INF MODEL JI J. Chem Inf. Model. PD NOV PY 2012 VL 52 IS 11 BP 2902 EP 2909 DI 10.1021/ci300289b PG 8 WC Chemistry, Medicinal; Chemistry, Multidisciplinary; Computer Science, Information Systems; Computer Science, Interdisciplinary Applications SC Pharmacology & Pharmacy; Chemistry; Computer Science GA 042HD UT WOS:000311461400011 PM 23036090 ER PT J AU Cawkwell, MJ Sanville, EJ Mniszewski, SM Niklasson, AMN AF Cawkwell, M. J. Sanville, E. J. Mniszewski, S. M. Niklasson, Anders M. N. TI Computing the Density Matrix in Electronic Structure Theory on Graphics Processing Units SO JOURNAL OF CHEMICAL THEORY AND COMPUTATION LA English DT Article ID TIGHT-BINDING; QUANTUM-CHEMISTRY; 1ST PRINCIPLES; DIAGONALIZATION AB The Self-consistent solution of a Schrodinger-like equation for the density matrix is a critical and computationally demanding step in quantum based models of interatomic bonding. This step was tackled historically via the diagonalization of the Hamiltonian. We have investigated the performance and accuracy of the second-order spectral projection (SP2) algorithm for the computation of the density matrix via a recursive expansion of the Fermi operator in a series of generalized matrix-matrix multiplications. We demonstrate that owing to its simplicity, the SP2 algorithm [Niklasson, A. M. N. Phys. Rev. B 2002, 66, 155115] is exceptionally well suited to implementation on graphics processing units (GPUs). The performance in double and single precision arithmetic of a hybrid GPU/central processing unit (CPU), and full GPU implementation of the SP2 algorithm exceed those of a CPU only implementation of the SP2 algorithm and traditional matrix diagonalization when the dimensions of the matrices exceed about 2000 x 2000. Padding schemes for arrays allocated hi the GPU memory that optimize the performance. Of the CUBLAS implementations of the level 3 BLAS DGEMM and SGEMM subroutines for generalized matrix-matrix multiplications are described in detail. The analysis Of the relative performance of the hybrid CPU/GPU and full GPU implementations indicate that the transfer of arrays between the GPU and CPU constitutes only a small fraction Of the total computation time The errors measured in the self consistent density matrices computed using the SP2 algorithm are generally smaller than those measured in matrices computed via diagonalization. Furthermore, the errors in the density matrices computed using the SP2 algorithm do not exhibit any dependence of system size, whereas the errors increase linearly with the number of orbitals when diagonalization is employed. C1 [Cawkwell, M. J.; Sanville, E. J.; Niklasson, Anders M. N.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Mniszewski, S. M.] Los Alamos Natl Lab, Comp Computat & Stat Sci Div, Los Alamos, NM 87545 USA. RP Cawkwell, MJ (reprint author), Los Alamos Natl Lab, Div Theoret, POB 1663, Los Alamos, NM 87545 USA. EM cawkwell@lanl.gov OI Mniszewski, Susan/0000-0002-0077-0537; Cawkwell, Marc/0000-0002-8919-3368 FU LDRD program at Los Alamos National Laboratory FX We thank Nick Bock, Kyle Spafford, and Jeffrey Vetter for stimulating discussions. This work was supported by the LDRD program at Los Alamos National Laboratory. NR 32 TC 10 Z9 10 U1 0 U2 25 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1549-9618 EI 1549-9626 J9 J CHEM THEORY COMPUT JI J. Chem. Theory Comput. PD NOV PY 2012 VL 8 IS 11 BP 4094 EP 4101 DI 10.1021/ct300442w PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 038RN UT WOS:000311191900012 PM 26605576 ER PT J AU Jiang, W Luo, Y Maragliano, L Roux, B AF Jiang, Wei Luo, Yun Maragliano, Luca Roux, Benoit TI Calculation of Free Energy Landscape in Multi-Dimensions with Hamiltonian-Exchange Umbrella Sampling on Petascale Supercomputer SO JOURNAL OF CHEMICAL THEORY AND COMPUTATION LA English DT Article ID HISTOGRAM ANALYSIS METHOD; MOLECULAR-DYNAMICS; CALBINDIN D-9K; LIGAND-BINDING; EF-HANDS; SIMULATIONS; EFFICIENCY; PROGRAM; CHARMM; FLUID AB An extremely scalable computational strategy is described for calculations of the potential of mean force (PMF) in multidimensions on massively distributed supercomputers. The approach involves coupling thousands of umbrella sampling (US) simulation windows distributed to cover the space of order parameters with a Hamiltonian molecular dynamics replica exchange (H-REMD) algorithm to enhance the sampling of each simulation. In the present application, US/H-REMD is carried out in,a two-dimensional (2D) space and exchanges are attempted alternatively along the two axes corresponding to the two order parameters. The US/H-REMD strategy is implemented on the basis of parallel/parallel multiple copy protocol at the MPI level, and therefore can fully exploit computing power of large-scale supercomputers. Here the novel technique is illustrated using the leadership supercomputer IBM Blue Gene/P with an application to a typical biomolecular calculation of general interest, namely the binding of calcium ions to the small protein Calbindin D-9k. The free energy landscape associated with two order parameters, the distance between the ion and its binding pocket and the root-mean-square deviation (rmsd) of the binding pocket relative the crystal structure, was calculated using the US/H-REMD method. The results are then used to estimate the absolute binding free energy of calcium ion to Calbindin D-9k. The tests demonstrate that the 2D US/H-REMD scheme greatly accelerates the configurational sampling of the binding pocket, thereby improving the convergence of the potential of mean force calculation. C1 [Jiang, Wei; Luo, Yun; Roux, Benoit] Argonne Natl Lab, Argonne Leadership Comp Facil, Argonne, IL 60439 USA. Argonne Natl Lab, Biosci Div, Argonne, IL 60439 USA. [Maragliano, Luca; Roux, Benoit] Univ Chicago, Gordon Ctr Integrat Sci, Dept Biochem & Mol Biol, Chicago, IL 60637 USA. RP Roux, B (reprint author), Argonne Natl Lab, Argonne Leadership Comp Facil, 9700 S Cass Ave,Bldg 240, Argonne, IL 60439 USA. EM roux@uchicago.edu RI Maragliano, Luca/A-8294-2010 OI Maragliano, Luca/0000-0002-5705-6967 FU National Science Foundation [MCB-0920261]; Computational Postdoctoral Fellowship of Argonne Leadership Computing Facility (ALCF); Early Science Postdoctoral Fellowship for Blue Gene/Q of ALCF; Office of Science of the U.S. Department of Energy [DE-AC02-06CH11357] FX We are grateful to Dr. Andrew Binkowski for his support. This research is funded by Grant MCB-0920261 from the National Science Foundation. W.J.'s research was supported by the Computational Postdoctoral Fellowship of Argonne Leadership Computing Facility (ALCF). Y.L.'s research is supported by the Early Science Postdoctoral Fellowship for Blue Gene/Q of ALCF. This research used the ALCF resource at ANL, which is supported by the Office of Science of the U.S. Department of Energy under Contract DE-AC02-06CH11357. NR 34 TC 32 Z9 32 U1 1 U2 36 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1549-9618 EI 1549-9626 J9 J CHEM THEORY COMPUT JI J. Chem. Theory Comput. PD NOV PY 2012 VL 8 IS 11 BP 4672 EP 4680 DI 10.1021/ct300468g PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 038RN UT WOS:000311191900067 PM 26605623 ER PT J AU Remillard, J Kollias, P Luke, E Wood, R AF Remillard, Jasmine Kollias, Pavlos Luke, Edward Wood, Robert TI Marine Boundary Layer Cloud Observations in the Azores SO JOURNAL OF CLIMATE LA English DT Article ID SOUTHEAST PACIFIC STRATOCUMULUS; RADIATIVELY DRIVEN CONVECTION; LIQUID WATER PATH; TURBULENCE STRUCTURE; CUMULUS CONVECTION; RADAR OBSERVATIONS; STRATIFORM CLOUDS; SEASONAL CYCLE; DIURNAL CYCLE; DOPPLER RADAR AB The recent deployment of the Atmospheric Radiation Measurement Program (ARM) Mobile Facility at Graciosa Island, Azores, in the context of the Clouds, Aerosol and Precipitation in the Marine Boundary Layer (CAP-MBL) field campaign added the most extensive (19 months) and comprehensive dataset of marine boundary layer (MBL) clouds to date. Cloud occurrence is high (60%-80%), with a summertime minimum. Liquid precipitation is frequently present (30%-40%), mainly in the form of virga. Boundary layer clouds are the most frequently observed cloud type (40%-50%) with a maximum of occurrence during the summer and fall months under the presence of anticyclonic conditions. Cumulus clouds are the most frequently occurring MBL cloud type (20%) with cumulus under stratocumulus layers (10%-30%) and single-layer stratocumulus (0%-10%) following in frequency of occurrence. A stable transition layer in the subcloud layer is commonly observed (92% of the soundings). Cumulus cloud bases and stratocumulus cloud tops correlate very well with the top of the transition layer and the inversion base, respectively. Drizzling stratocumulus layers are thicker (350-400 m) and have higher liquid water path (75-150 g m(-2)) than their nondrizzling counterparts (100-250 m and 30-75 g m(-2), respectively). The variance of the vertical air motion is maximum near the cloud base and is higher at night. The updraft mass flux is around 0.17 kg m(-2) s(-1) with 40%-60% explained by coherent updraft structures. Despite a high frequency of stratocumulus clouds in the Azores, the MBL is almost never well mixed and is often cumulus coupled. C1 [Remillard, Jasmine; Kollias, Pavlos] McGill Univ, Dept Atmospher & Ocean Sci, Montreal, PQ H3A 2K6, Canada. [Luke, Edward] Brookhaven Natl Lab, Div Atmospher Sci, Upton, NY 11973 USA. [Wood, Robert] Univ Washington, Dept Atmospher Sci, Seattle, WA 98195 USA. RP Remillard, J (reprint author), McGill Univ, Dept Atmospher & Ocean Sci, Room 945,Burnside Hall,805 Sherbrooke St W, Montreal, PQ H3A 2K6, Canada. EM jasmine.remillard@mail.mcgill.ca RI Wood, Robert/A-2989-2008 OI Wood, Robert/0000-0002-1401-3828 NR 61 TC 32 Z9 32 U1 2 U2 36 PU AMER METEOROLOGICAL SOC PI BOSTON PA 45 BEACON ST, BOSTON, MA 02108-3693 USA SN 0894-8755 J9 J CLIMATE JI J. Clim. PD NOV 1 PY 2012 VL 25 IS 21 BP 7381 EP 7398 DI 10.1175/JCLI-D-11-00610.1 PG 18 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 036BZ UT WOS:000311002700005 ER PT J AU Lu, J Zhao, B AF Lu, Jian Zhao, Bin TI The Role of Oceanic Feedback in the Climate Response to Doubling CO2 SO JOURNAL OF CLIMATE LA English DT Article ID FLUCTUATION-DISSIPATION THEOREM; HEMISPHERE ATMOSPHERIC CIRCULATION; SEA-SURFACE TEMPERATURE; INTERANNUAL VARIABILITY; SOUTHERN-HEMISPHERE; HYDROLOGICAL CYCLE; EL-NINO; MODEL; PACIFIC; CCSM3 AB Two suites of partial coupling experiments are devised with the upper-ocean dynamics version (UOM) of the CCSM3 to isolate the effects of the feedbacks from the change of the wind-driven ocean circulation and air-sea heat flux in the global climate response to the forcing of doubling CO2. The partial coupling is achieved by implementing a so-called overriding technique, which helps quantitatively partition the total response in the fully coupled model to the feedback component in question and the response to external forcing in the absence of the former. By overriding the wind stress seen by the ocean and the wind speed through the bulk formula for evaporation, the experiments help to reveal that (i) the wind-evaporation-SST (WES) feedback is the main formation mechanism for the tropical SST pattern under the CO2 forcing, verifying the hypothesis proposed by Xie et al.; (ii) the weakened tropical Pacific wind is shown in this UOM model not to be the cause for the enhanced equatorial Pacific warming, as one might expect from the thermocline and Bjerknes feedbacks; (iii) WES is also the leading mechanism for shaping the tropical precipitation response in the ocean; and (iv) both the wind-driven ocean dynamical feedback and the WES feedback act to increase the persistence of the southern annular mode (SAM) and the increased time scale of the SAM due to these feedbacks manifests itself in the response of the jet shift to an identical CO2 forcing, in a manner conforming to the fluctuation-dissipation theorem. C1 [Lu, Jian] Ctr Ocean Land Atmosphere Studies, Inst Global Environm & Soc, Calverton, MD 20705 USA. [Lu, Jian] George Mason Univ, Dept Atmospher Ocean & Earth Sci, Fairfax, VA 22030 USA. [Zhao, Bin] NASA Goddard Space & Flight Ctr, Global Modeling & Assimilat Off, Camp Greenbelt, MD USA. [Zhao, Bin] Los Alamos Natl Lab, COSIM Project, Grp T3, Los Alamos, NM USA. RP Lu, J (reprint author), Ctr Ocean Land Atmosphere Studies, Inst Global Environm & Soc, 4041 Powder Mill Rd,Suite 302, Calverton, MD 20705 USA. EM jianlu@cola.iges.org FU COLA omnibus fund from NSF [830068]; NOAA [NA09OAR3210058]; NSF [AGS-1064045]; IGPP from the Los Alamos branch of the Institute of Geophysics and Planetary Physics [1544]; NASA [NNX09AN50G] FX The experiment design of this paper benefited greatly from the conversation with William Large and Clara Deser of NCAR. The authors are grateful to Gokhan Danabasoglu for providing the data of the long integrations with the full CCSM3-FDM. Gang Chen suggested the analysis of the lag-correlation time scale of the SAM and its relationship with the shift of the midlatitude westerlies. Comments from Shang-Ping Xie on the early version of manuscript are also gratefully acknowledged. Comments from three anonymous reviewers helped improve the manuscript substantially. Discussion with Edwin Schneider and Ben Kirtman helped us understand the bias caused by the wind overriding. V. Krishnamurthy and Abraham Solomon provided editorial assistance during the revision of the manuscript. This research is supported by the COLA omnibus fund from NSF Grant 830068, NOAA Grant NA09OAR3210058, and NASA Grant NNX09AN50G. J. Lu is also partially supported by the NSF Grant AGS-1064045. The experiments were conducted by B. Zhao when he was a postdoctoral research scientist at Los Alamos National Laboratory, supported by IGPP Award 1544 from the Los Alamos branch of the Institute of Geophysics and Planetary Physics. NR 54 TC 25 Z9 25 U1 1 U2 19 PU AMER METEOROLOGICAL SOC PI BOSTON PA 45 BEACON ST, BOSTON, MA 02108-3693 USA SN 0894-8755 EI 1520-0442 J9 J CLIMATE JI J. Clim. PD NOV 1 PY 2012 VL 25 IS 21 BP 7544 EP 7563 DI 10.1175/JCLI-D-11-00712.1 PG 20 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 036BZ UT WOS:000311002700013 ER PT J AU Murphy, LN Riley, WJ Collins, WD AF Murphy, Lisa N. Riley, William J. Collins, William D. TI Local and Remote Climate Impacts from Expansion of Woody Biomass for Bioenergy Feedstock in the Southeastern United States SO JOURNAL OF CLIMATE LA English DT Article ID LAND-COVER CHANGE; NORTH-ATLANTIC OSCILLATION; LOBLOLLY-PINE; TEMPERATURE; VARIABILITY; FORESTS; CARBON; DYNAMICS; FIELD; SIMULATIONS AB Many efforts have been taken to find energy alternatives to reduce anthropogenic influences on climate. Recent studies have shown that using land for bioenergy plantations may be more cost effective and provide a greater potential for CO2 abatement than using land for carbon sequestration. Native southern U.S. pines (i.e., loblolly) have excellent potential as bioenergy feedstocks. However, the land-cover change due to expansion of biofuels may impact climate through biophysical feedbacks. Here. the authors access the local and remote consequences of greater forest management and biofuel feedstock expansion on climate and hydrology using a global climate model, the NCAR Community Climate System Model, version 4 (CCSM4). The authors examine a plausible U.S. Department of Energy (DOE) biofuel feedstock goal by afforesting 50 million acres of C-4 grasslands in the southeastern United States with an optimized loblolly plant functional type. Changes in sensible and latent heat fluxes are related to increased surface roughness, reduced bare-ground evaporation, and changes in stomatal conductance. In the coupled simulations, these mechanisms lead to a 1 degrees C cooling, higher atmospheric stability, and a more shallow planetary boundary layer over the southeastern United States during the summer; in winter, a cooling of up to 0.25 degrees C between 40 degrees and 60 degrees N, a weakened Aleutian low, and a wetter Australia occurs. A weakened Aleutian low shifts the North Pacific storm track poleward in the future loblolly scenarios. These local and global impacts suggest that biophysical feedbacks need to be considered when evaluating the benefits of bioenergy feedstock production. C1 [Murphy, Lisa N.; Riley, William J.; Collins, William D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Climate Sci Dept, Berkeley, CA 94720 USA. [Collins, William D.] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. RP Murphy, LN (reprint author), Univ Miami, 4600 Rickenbacker Causeway, Miami, FL 33149 USA. EM lmurphy@rsmas.miami.edu RI Murphy, Lisa/B-8547-2013; Collins, William/J-3147-2014; Riley, William/D-3345-2015 OI Murphy, Lisa/0000-0003-4343-8005; Collins, William/0000-0002-4463-9848; Riley, William/0000-0002-4615-2304 FU Office of Science, Office of Biological and Environmental Research of the U.S. Department of Energy [DE-AC02-05CH11231] FX This research was supported by the Director, Office of Science, Office of Biological and Environmental Research of the U.S. Department of Energy under Contract DE-AC02-05CH11231 as part of their Climate and Earth System Modeling Program. NR 63 TC 2 Z9 2 U1 0 U2 27 PU AMER METEOROLOGICAL SOC PI BOSTON PA 45 BEACON ST, BOSTON, MA 02108-3693 USA SN 0894-8755 J9 J CLIMATE JI J. Clim. PD NOV 1 PY 2012 VL 25 IS 21 BP 7643 EP 7659 DI 10.1175/JCLI-D-11-00535.1 PG 17 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 036BZ UT WOS:000311002700019 ER PT J AU Xie, SC Ma, HY Boyle, JS Klein, SA Zhang, YY AF Xie, Shaocheng Ma, Hsi-Yen Boyle, James S. Klein, Stephen A. Zhang, Yuying TI On the Correspondence between Short- and Long-Time-Scale Systematic Errors in CAM4/CAM5 for the Year of Tropical Convection SO JOURNAL OF CLIMATE LA English DT Article ID COMMUNITY-ATMOSPHERE-MODEL; GENERAL-CIRCULATION MODELS; CLIMATE SIMULATIONS; WEATHER PREDICTION; VERSION-3 CAM3; CLOUDS; IMPACT; SATELLITE; PARAMETERIZATION; REPRESENTATION AB The correspondence between short-and long-time-scale systematic errors in the Community Atmospheric Model, version 4 (CAM4) and version 5 (CAM5), is systematically examined. The analysis is based on the annual-mean data constructed from long-term "free running" simulations and short-range hindcasts. The hindcasts are initialized every day with the ECMWF analysis for the Year(s) of Tropical Convection. It has been found that most systematic errors, particularly those associated with moist processes, are apparent in day 2 hindcasts. These errors steadily grow with the hindcast lead time and typically saturate after five days with amplitudes comparable to the climate errors. Examples include the excessive precipitation in much of the tropics and the overestimate of net shortwave absorbed radiation in the stratocumulus cloud decks over the eastern subtropical oceans and the Southern Ocean at about 60 degrees S. This suggests that these errors are likely the result of model parameterization errors as the large-scale flow remains close to observed in the first few days of the hindcasts. In contrast, other climate errors are present in the hindcasts, but with amplitudes that are significantly smaller than and do not approach their climate errors during the 6-day hindcasts. These include the cold biases in the lower stratosphere, the unrealistic double-intertropical convergence zone pattern in the simulated precipitation, and an annular mode bias in extratropical sea level pressure. This indicates that these biases could be related to slower processes such as radiative and chemical processes, which are important in the lower stratosphere, or the result of poor interactions of the parameterized physics with the large-scale flow. C1 [Xie, Shaocheng] Lawrence Livermore Natl Lab, Atmospher Earth & Energy Div L 103, Livermore, CA 94550 USA. RP Xie, SC (reprint author), Lawrence Livermore Natl Lab, Atmospher Earth & Energy Div L 103, POB 808, Livermore, CA 94550 USA. EM xie2@llnl.gov RI Ma, Hsi-Yen/K-1019-2013; Xie, Shaocheng/D-2207-2013; Zhang, Yuying/H-5011-2012; Klein, Stephen/H-4337-2016 OI Xie, Shaocheng/0000-0001-8931-5145; Klein, Stephen/0000-0002-5476-858X FU Office of Science at the U.S. Department of Energy; U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work is supported by the Regional and Global Climate Modeling Program and Atmospheric System Research Program of the Office of Science at the U.S. Department of Energy. Work at LLNL was performed under the auspices of the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 37 TC 27 Z9 27 U1 1 U2 23 PU AMER METEOROLOGICAL SOC PI BOSTON PA 45 BEACON ST, BOSTON, MA 02108-3693 USA SN 0894-8755 EI 1520-0442 J9 J CLIMATE JI J. Clim. PD NOV PY 2012 VL 25 IS 22 BP 7937 EP 7955 DI 10.1175/JCLI-D-12-00134.1 PG 19 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 036NO UT WOS:000311034300010 ER PT J AU Muth, D Bryden, KM AF Muth, D., Jr. Bryden, K. M. TI A Conceptual Evaluation of Sustainable Variable-Rate Agricultural Residue Removal SO JOURNAL OF ENVIRONMENTAL QUALITY LA English DT Article ID SOIL ORGANIC-CARBON; CORN STOVER HARVEST; MANAGEMENT; EROSION; METHODOLOGY; WHEAT AB Agricultural residues have near-term potential as a feedstock for bioenergy production, but their removal must be managed carefully to maintain soil health and productivity. Recent studies have shown that subfield scale variability in soil properties (e.g., slope, texture, and organic matter content) that affect grain yield significantly affect the amount of residue that can be sustainably removed from different areas within a single field. This modeling study examines the concept of variable-rate residue removal equipment that would be capable of on-the-fly residue removal rate adjustments ranging from 0 to 80%. Thirteen residue removal rates (0% and 25-80% in 5% increments) were simulated using a subfield scale integrated modeling framework that evaluates residue removal sustainability considering wind erosion, water erosion, and soil carbon constraints. Three Iowa fields with diverse soil, slope, and grain yield characteristics were examined and showed sustainable, variable-rate agricultural residue removal that averaged 2.35, 7.69, and 5.62 Mg ha(-1), respectively. In contrast, the projected sustainable removal rates using rake and bale removal for the entire field averaged 0.0, 6.40, and 5.06 Mg ha(-1), respectively. The modeling procedure also projected that variable-rate residue harvest would result in 100% of the land area in all three fields being managed in a sustainable manner, whereas Field 1 could not be sustainably managed using rake and bale removal, and only 83 and 62% of the land area in Fields 2 and 3 would be managed sustainably using a rake and bale operation for the entire field. In addition, it was found that residue removal adjustments of 40 to 65% are sufficient to collect 90% of the sustainably available agricultural residue. C1 [Muth, D., Jr.] Idaho Natl Lab, Biofuels & Renewable Energy Technol Div, Idaho Falls, ID 83415 USA. [Bryden, K. M.] Ames Lab, Simulat Modeling & Decis Sci Program, Ames, IA 50011 USA. RP Muth, D (reprint author), Idaho Natl Lab, Biofuels & Renewable Energy Technol Div, Idaho Falls, ID 83415 USA. EM David.Muth@inl.gov RI Bryden, Kenneth/G-6918-2012 FU DOE'S Office of the Biomass Program; DOE Biomass Regional Feedstock Partnership Program; MonsantoMike Edgerton; Sun Grant Initiative through the Biomass Regional Feedstock Partnership FX This work was funded in part by the DOE'S Office of the Biomass Program. The authors gratefully acknowledge the significant support from all partners in the DOE Biomass Regional Feedstock Partnership Program and Monsanto and Mike Edgerton for providing data and funding to execute the study analyses. The authors also gratefully acknowledge David Muth Sr. for providing study data. Professor Bryden gratefully acknowledges the funding support of the Sun Grant Initiative through the Biomass Regional Feedstock Partnership. NR 35 TC 4 Z9 4 U1 2 U2 30 PU AMER SOC AGRONOMY PI MADISON PA 677 S SEGOE RD, MADISON, WI 53711 USA SN 0047-2425 J9 J ENVIRON QUAL JI J. Environ. Qual. PD NOV-DEC PY 2012 VL 41 IS 6 BP 1796 EP 1805 DI 10.2134/jeq2012.0067 PG 10 WC Environmental Sciences SC Environmental Sciences & Ecology GA 039QU UT WOS:000311262400011 PM 23128737 ER PT J AU Yang, J Hong, KL Bonnesen, PV AF Yang, Jun Hong, Kunlun Bonnesen, Peter V. TI Synthesis of N1-tritylethane-1,1,2,2-d4-1,2-diamine: a novel mono-protected C-deuterated ethylenediamine synthon SO JOURNAL OF LABELLED COMPOUNDS & RADIOPHARMACEUTICALS LA English DT Article DE deuterated ethylenediamine; ethylenediamine-C-d4; trityl-protected ethylenediamine-C-d4; en-C-d4; Mitsunobu reaction ID DIAMINES AB A convenient and high-yield synthesis for N1-tritylethane-1,1,2,2-d4-1,2-diamine, a novel mono-protected ethylenediamine-C-d4, is reported. N1-tritylethane-1,1,2,2-d4-1,2-diamine was prepared in three steps from ethylene oxide-d4 in a combined yield in the range 6876%. Also reported is a synthesis of ethylenediamine-C-d4 in two steps from 1,2-dibromoethane-d4 in a combined yield in the range 6165%. C1 [Yang, Jun; Hong, Kunlun; Bonnesen, Peter V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Bonnesen, PV (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM bonnesenpv@ornl.gov RI Bonnesen, Peter/A-1889-2016; Hong, Kunlun/E-9787-2015 OI Bonnesen, Peter/0000-0002-1397-8281; Hong, Kunlun/0000-0002-2852-5111 FU Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy; US Department of Energy [DE-AC05-00OR22725] FX This research was conducted at the Center for Nanophase Materials Sciences, which is sponsored at the Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. This manuscript has been authored by UT-Battelle, LLC, under Contract No. DE-AC05-00OR22725 with the US Department of Energy. The publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. NR 14 TC 1 Z9 1 U1 0 U2 11 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0362-4803 J9 J LABELLED COMPD RAD JI J. Label. Compd. Radiopharm. PD NOV PY 2012 VL 55 IS 13 BP 463 EP 466 DI 10.1002/jlcr.2977 PG 4 WC Biochemical Research Methods; Chemistry, Medicinal; Chemistry, Analytical SC Biochemistry & Molecular Biology; Pharmacology & Pharmacy; Chemistry GA 041MU UT WOS:000311406700004 ER PT J AU Millett, PC Zhang, YF Andersson, DA Tonks, MR Biner, SB AF Millett, Paul C. Zhang, Yongfeng Andersson, D. A. Tonks, Michael R. Biner, S. B. TI Random-walk Monte Carlo simulation of intergranular gas bubble nucleation in UO2 fuel SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID GRAIN-BOUNDARY SEGREGATION; FISSION-GAS; SURFACE SEGREGATION; KINETICS; GROWTH; DIFFUSION; MODEL; RELEASE; MIGRATION; METALS AB Using a random-walk particle algorithm, we investigate the clustering of fission gas atoms on grain boundaries in oxide fuels. The computational algorithm implemented in this work considers a planar surface representing a grain boundary on which particles appear at a rate dictated by the Booth flux, migrate two dimensionally according to their grain boundary diffusivity, and coalesce by random encounters. Specifically, the intergranular bubble nucleation density is the key variable we investigate using a parametric study in which the temperature, grain boundary gas diffusivity, and grain boundary segregation energy are varied. The results reveal that the grain boundary bubble nucleation density can vary widely due to these three parameters, which may be an important factor in the observed variability in intergranular bubble percolation among grain boundaries in oxide fuel during fission gas release. Published by Elsevier B.V. C1 [Millett, Paul C.; Zhang, Yongfeng; Tonks, Michael R.; Biner, S. B.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. [Andersson, D. A.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Millett, PC (reprint author), Idaho Natl Lab, Idaho Falls, ID 83415 USA. EM Paul.Millett@inl.gov FU Nuclear Energy Modeling and Simulation (NEAMS) FX The authors gratefully acknowledge financial support from the Nuclear Energy Modeling and Simulation (NEAMS), and specifically the Fundamental Models and Methods (FMM), Programs within the US Department of Energy. NR 25 TC 0 Z9 0 U1 2 U2 17 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 J9 J NUCL MATER JI J. Nucl. Mater. PD NOV PY 2012 VL 430 IS 1-3 BP 44 EP 49 DI 10.1016/j.jnucmat.2012.06.049 PG 6 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA 035IT UT WOS:000310940700007 ER PT J AU Kim, YS Park, JM Ryu, HJ Jung, YH Hofman, GL AF Kim, Yeon Soo Park, Jong Man Ryu, Ho Jin Jung, Yang Hong Hofman, G. L. TI Reduced interaction layer growth of U-Mo dispersion in Al-Si SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID FUEL; ALLOY; INTERDIFFUSION; IRRADIATION; PRODUCT AB Development of high U-density U-Mo fuel particle dispersion in Al is needed to convert high power research and test reactors from HEU to LEU. Interaction layer growth between U-Mo and Al poses a challenge to this goal. The KOMO-4 test was designed at KAERI and irradiated in the HANARO reactor to similar to 50% burnup of initial 19.75% U-235 enrichment at similar to 200 degrees C. The main objective of the test was to examine the effect of the Si content in the matrix up to 8 wt.%. U-Mo/Al-Si dispersion samples with a Si addition in the range 0-8 wt.% in the matrix were tested. A sample with pre-irradiation Si-containing interaction layers (ILs) was also tested. As the Si content in the matrix increases, the IL growth was progressively reduced. Contrary to the thermodynamics prediction and out-of-pile observations, however, Si accumulation in the ILs occurred near the IL-matrix interface with only a slight increase in concentration. The effect of the pre-formed ILs was insignificant in reducing IL growth. (C) 2012 Elsevier B.V. All rights reserved. C1 [Kim, Yeon Soo; Hofman, G. L.] Argonne Natl Lab, Argonne, IL 60439 USA. [Park, Jong Man; Ryu, Ho Jin; Jung, Yang Hong] Korea Atom Energy Res Inst, Taejon 305353, South Korea. RP Kim, YS (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. EM yskim@anl.gov RI RYU, HO JIN/J-2764-2013 OI RYU, HO JIN/0000-0002-3387-7381 FU US Department of Energy, Office of Global Threat Reduction (NA-21), National Nuclear Security Administration [DE-AC-02-06CH11357]; National Nuclear R&D Program of the Korean Ministry of Education, Science and Technology (MEST) FX The authors are grateful to Mr. B.O. Yoo for the PIE work of KOMO-4 test samples and to Dr. H.T. Chae and Dr. C.G. Seo for the physics and safety analyses of the KOMO-4 irradiation test. The operations staffs at HANARO (KAERI) are also acknowledged for the test. One of the authors (Y.S. Kim) appreciates the comments by Ms. S.H. Kim of Cambridge, MA. KAERI's work was supported by the National Nuclear R&D Program of the Korean Ministry of Education, Science and Technology (MEST). This work was supported in part by the US Department of Energy, Office of Global Threat Reduction (NA-21), National Nuclear Security Administration, under Contract No. DE-AC-02-06CH11357 between UChicago Argonne, LLC and the Department of Energy. NR 51 TC 11 Z9 11 U1 1 U2 8 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 J9 J NUCL MATER JI J. Nucl. Mater. PD NOV PY 2012 VL 430 IS 1-3 BP 50 EP 57 DI 10.1016/j.jnucmat.2012.06.032 PG 8 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA 035IT UT WOS:000310940700008 ER PT J AU Zhang, YF Liu, XY Millett, PC Tonks, M Andersson, DA Biner, B AF Zhang, Yongfeng Liu, Xiang-Yang Millett, Paul C. Tonks, Michael Andersson, David A. Biner, Bulent TI Crack tip plasticity in single crystal UO2: Atomistic simulations SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID MOLECULAR-DYNAMICS SIMULATION; DENSITY-FUNCTIONAL THEORY; SINTERED URANIUM-DIOXIDE; INTERATOMIC POTENTIALS; FRACTURE-TOUGHNESS; HIGH-TEMPERATURES; SURFACE-ENERGY; FUEL PELLETS; TRANSFORMATION; STRENGTH AB The fracture behavior of single crystal uranium dioxide under mode-I loading is studied using molecular dynamics simulations at room temperature. The initial cracks are introduced as elliptical notches on either {1 1 1} or {1 1 0} planes. Two crack tip shielding mechanisms, dislocation emission and metastable phase transformation are identified. Crack extension is observed for cracks residing on {1 1 1} plane only. The dislocations have a Burgers vector of < 1 1 0 >/2 and glide on {1 0 0} planes. Two metastable phases. Rutile and Scrutinyite, are identified during the phase transformation, and their relative stability is confirmed by separate density-functional-theory calculations. Examination of stress field near the crack tips reveals that dislocation emission is not as an effective shielding mechanism as the phase transformation. The formation of new phases may effectively shield the crack if all phase interfaces formed near the crack tips are coherent, as in the case of cracks residing on {1 1 0} planes. (C), 2012 Elsevier B.V. All rights reserved. C1 [Zhang, Yongfeng; Millett, Paul C.; Tonks, Michael; Biner, Bulent] Idaho Natl Lab, Idaho Falls, ID 83415 USA. [Liu, Xiang-Yang; Andersson, David A.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Zhang, YF (reprint author), Idaho Natl Lab, Idaho Falls, ID 83415 USA. EM yongfeng.zhang@inl.gov FU DOE [FTLA11MS0603] FX The authors gratefully acknowledge the support of the DOE Nuclear Energy Advanced Modeling and Simulation (NEAMS) Program, under the Fuels Integrated Performance and Safety Code (IPSC) project with work Package No. FTLA11MS0603. Yongfeng Zhang thanks Drs. Blas Uberuaga and Richard Hoagland for beneficial discussions. NR 52 TC 8 Z9 9 U1 3 U2 26 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD NOV PY 2012 VL 430 IS 1-3 BP 96 EP 105 DI 10.1016/j.jnucmat.2012.06.044 PG 10 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA 035IT UT WOS:000310940700014 ER PT J AU Chockalingam, K Millett, PC Tonks, MR AF Chockalingam, K. Millett, Paul C. Tonks, M. R. TI Effects of intergranular gas bubbles on thermal conductivity SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID GRAIN-BOUNDARIES; RESISTANCE; SIMULATION; KINETICS AB Model microstructures obtained from phase-field simulations are used to study the effective heat transfer across bicrystals with stationary grain boundary bubble populations. We find that the grain boundary coverage, irrespective of the intergranular bubble radii, is the most relevant parameter to the thermal resistance, which we use to derive effective Kapitza resistances that are dependent on the grain boundary coverage and Kaptiza resistance of the intact grain boundary. We propose a model to predict thermal conductivity as a function of porosity, grain-size, Kaptiza resistance of the intact grain boundary, and grain boundary bubble coverage. Published by Elsevier B.V. C1 [Chockalingam, K.; Millett, Paul C.; Tonks, M. R.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. RP Chockalingam, K (reprint author), Idaho Natl Lab, POB 1625, Idaho Falls, ID 83415 USA. EM Karthikeyan.Chockalingam@inl.gov; Paul.Millett@inl.gov; Michael.Tonks@inl.gov FU Nuclear Energy Modeling and Simulation (NEAMS) program within the US Department of Energy FX The authors thank Dr. S.B. Biner of Idaho National Laboratory for reviewing the manuscript before it's submission. The authors gratefully acknowledge financial support from the Nuclear Energy Modeling and Simulation (NEAMS) program within the US Department of Energy. NR 15 TC 12 Z9 12 U1 4 U2 23 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 J9 J NUCL MATER JI J. Nucl. Mater. PD NOV PY 2012 VL 430 IS 1-3 BP 166 EP 170 DI 10.1016/j.jnucmat.2012.06.027 PG 5 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA 035IT UT WOS:000310940700024 ER PT J AU Besmann, TM Stoller, RE Samolyuk, G Schuck, PC Golubov, SI Rudin, SP Wills, JM Coe, JD Wirth, BD Kim, S Morgan, DD Szlufarska, I AF Besmann, T. M. Stoller, R. E. Samolyuk, G. Schuck, P. C. Golubov, S. I. Rudin, S. P. Wills, J. M. Coe, J. D. Wirth, B. D. Kim, S. Morgan, D. D. Szlufarska, I. TI Modeling Deep Burn TRISO particle nuclear fuel SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID FISSION-PRODUCT RELEASE; GAS-COOLED REACTORS; RESEARCH-AND-DEVELOPMENT; AUGMENTED-WAVE METHOD; THERMAL-CONDUCTIVITY; OXYGEN SYSTEM; INTERFACE REACTIONS; KERNEL MIGRATION; SILICON-CARBIDE; POINT-DEFECTS AB Under the DOE Deep Burn program TRISO fuel is being investigated as a fuel form for consuming plutonium and minor actinides, and for greater efficiency in uranium utilization. The result will thus be to drive TRISO particulate fuel to very high burn-ups. In the current effort the various phenomena in the TRISO particle are being modeled using a variety of techniques. The chemical behavior is being treated utilizing thermochemical analysis to identify phase formation/transformation and chemical activities in the particle, including kernel migration. Density functional theory is being used to understand fission product diffusion within the plutonia oxide kernel, the fission product's attack on the SiC coating layer, as well as fission product diffusion through an alternative coating layer, ZrC. Finally, a multiscale approach is being used to understand thermal transport, including the effect of radiation damage induced defects, in a model SiC material. (C) 2012 Elsevier B.V. All rights reserved. C1 [Besmann, T. M.; Stoller, R. E.; Samolyuk, G.; Schuck, P. C.; Golubov, S. I.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Wirth, B. D.] Univ Tennessee, Knoxville, TN 37996 USA. [Rudin, S. P.; Wills, J. M.; Coe, J. D.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Kim, S.; Morgan, D. D.; Szlufarska, I.] Univ Wisconsin, Madison, WI 53706 USA. RP Besmann, TM (reprint author), Oak Ridge Natl Lab, POB 2008, Oak Ridge, TN 37831 USA. EM besmanntm@ornl.gov; stollerre@ornl.gov; samolyukgd@ornl.gov; schuckpc@ornl.gov; golubovsi@ornl.gov; srudin@lanl.gov; jxw@lanl.gov; jcoe@lanl.gov; bdwirth@utk.edu; sungtae@cae.wisc.e-du; ddmorgan@engr.wisc.edu; izabela@engr.wisc.edu RI Wirth, Brian/O-4878-2015 OI Wirth, Brian/0000-0002-0395-0285 FU U.S. Department of Energy [DE-AC05-00OR22725]; U.S. Department of Energy NE Deep Burn program FX This manuscript has been authored by UT-Battelle, LLC, under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up. irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes.; This work was funded under the U.S. Department of Energy NE Deep Burn program. The authors wish to thank T.R. Allen, S.L. Volt, and Y. Katoh for helpful discussions. K.T. Clarno performed the SCALE calculations. NR 66 TC 8 Z9 8 U1 2 U2 32 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 J9 J NUCL MATER JI J. Nucl. Mater. PD NOV PY 2012 VL 430 IS 1-3 BP 181 EP 189 DI 10.1016/j.jnucmat.2012.06.041 PG 9 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA 035IT UT WOS:000310940700026 ER PT J AU Anderoglu, O Van den Bosch, J Hosemann, P Stergar, E Sencer, BH Bhattacharyya, D Dickerson, R Dickerson, P Hartl, M Maloy, SA AF Anderoglu, O. Van den Bosch, J. Hosemann, P. Stergar, E. Sencer, B. H. Bhattacharyya, D. Dickerson, R. Dickerson, P. Hartl, M. Maloy, S. A. TI Phase stability of an HT-9 duct irradiated in FFTF SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID FERRITIC-MARTENSITIC STEELS; NEUTRON-SCATTERING; FAST-REACTOR; ALLOYS; SIMILAR-TO-400-DEGREES-C; RADIATION; BEHAVIOR; SYSTEM; CREEP; RATIO AB A fuel test assembly known as the ACO-3 duct made out of a normalized and fully tempered ferritic/martensitic steel (HT-9) was previously irradiated in the Fast Flux Test Reactor Facility (FFTF) up to 155 dpa at a temperature range of 380-504 degrees C. The microstructures of the samples from five different zones along a face of the duct were analyzed using a combination of transmission electron microscopy (TEM) based techniques, small angle neutron scattering (SANS) and atom probe tomography (APT). A high density of Cr rich alpha' precipitates together with a moderate density of G-phase precipitates with average sizes of similar to 4 and 11 nm respectively were found in the 20 dpa, 380 degrees C.zone. It was found that precipitation of the second phases is more sensitive to the temperature history then to the exposed neutron dose. In general, the density of both precipitates decreases with increasing irradiation temperature. No significant change is observed in average size of a' while the average size of G-phase precipitates increases up to 27 nm at 440 degrees C. Voids are observed after irradiation at 100 dpa (irradiation temperature of 410 degrees C) and 155 dpa (irradiation temperature of 440 degrees C) but no voids were detected after irradiation to 96 dpa (irradiation temperature of 466 degrees C). In contrast to what is previously reported in the literature, no Laves, M6C or Chi phases were found in any of the zones. Published by Elsevier B.V. C1 [Anderoglu, O.; Van den Bosch, J.; Hosemann, P.; Dickerson, R.; Dickerson, P.; Hartl, M.; Maloy, S. A.] Los Alamos Natl Lab, Los Alamos, NM 87544 USA. [Van den Bosch, J.; Stergar, E.] SCK CEN, B-2400 Mol, Belgium. [Hosemann, P.; Stergar, E.] Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA. [Sencer, B. H.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. [Bhattacharyya, D.] ANSTO, Inst Mat Engn, Lucas Heights, NSW 2234, Australia. RP Anderoglu, O (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87544 USA. EM oanderoglu@gmail.com RI Dickerson, Robert/C-9237-2013; Lujan Center, LANL/G-4896-2012; Hartl, Monika/F-3094-2014; Maloy, Stuart/A-8672-2009; Hartl, Monika/N-4586-2016; OI Hartl, Monika/0000-0002-6601-7273; Maloy, Stuart/0000-0001-8037-1319; Hartl, Monika/0000-0002-6601-7273; Hosemann, Peter/0000-0003-2281-2213 FU DOE-NE's Fuel Cycle Research and Development program; U.S. DOE NE under Idaho Operations Office Contract [DE-AC07-051D14517]; NRC faculty development grant [38-09-948]; Department of Energy's Office of Basic Energy Sciences; Los Alamos National Security LLC under DOE [DE-AC52-06NA25396] FX This research is funded by DOE-NE's Fuel Cycle Research and Development program. A portion of this research was supported by the U.S. DOE NE under Idaho Operations Office Contract DE-AC07-051D14517 and NRC faculty development grant-38-09-948. The authors would like to thank T. Romero for performing the hot cell work. We also acknowledge R.P. Hjelm for the help with the interpretation of SANS data. This work has benefitted from the use of the Manuel Lujan, Jr. Neutron Scattering Center at Los Alamos National Laboratory, which is funded by the Department of Energy's Office of Basic Energy Sciences. Los Alamos National laboratory is operated by Los Alamos National Security LLC under DOE Contract DE-AC52-06NA25396. NR 42 TC 13 Z9 13 U1 3 U2 31 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 J9 J NUCL MATER JI J. Nucl. Mater. PD NOV PY 2012 VL 430 IS 1-3 BP 194 EP 204 DI 10.1016/j.jnucmat.2012.06.038 PG 11 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA 035IT UT WOS:000310940700028 ER PT J AU Mihaila, B Stan, M Crapps, J AF Mihaila, Bogdan Stan, Marius Crapps, Justin TI Impact of thermal conductivity models on the coupling of heat transport and oxygen diffusion in UO2 nuclear fuel elements SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID THERMOPHYSICAL PROPERTIES; URANIUM-DIOXIDE; DEFECTIVE FUEL; SIMULATIONS; OXIDATION; RECOMMENDATIONS; EXPANSION; RODS; MOX AB We study the coupled thermal transport, oxygen diffusion, and thermal expansion of a generic nuclear fuel element consisting of a UO2 fuel pellet and stainless steel cladding separated by a helium gap for the purpose of evaluating the impact of various thermal conductivity models on the predictions of the temperature profile and deformation. Using a series of steady-state and time-dependent finite-element simulations with a variety of initial- and boundary-value conditions, thermo-mechanical response of the fuel element is evaluated. The results show that including the deviation from stoichiometry, x, in the thermal conductivity model is paramount for obtaining accurate predictions in the centerline temperature and the extent of the radial deformation of the fuel pellet. In a surprising result, the coupling between the heat transport and the oxygen diffusion is relatively strong for small values of the fixed composition boundary conditions x(b), whereas the coupling becomes weaker for large values of x(b). (C) 2012 Elsevier B.V. All rights reserved. C1 [Mihaila, Bogdan] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. [Stan, Marius; Crapps, Justin] Argonne Natl Lab, Nucl Engn Div, Argonne, IL 60439 USA. RP Mihaila, B (reprint author), Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. EM bmihaila@lanl.gov RI Mihaila, Bogdan/D-8795-2013 OI Mihaila, Bogdan/0000-0002-1489-8814 FU United States Department of Energy; Consortium for Advanced Simulation of Light Water Reactors; Energy Innovation Hub for Modeling and Simulation of Nuclear Reactors under US Department of Energy [DE-AC05-00OR22725]; US Department of Energy, Office of Science [DE-AC02-06CH11357] FX This work was performed under the auspices of the United States Department of Energy. BM gratefully acknowledges partial financial support from the Consortium for Advanced Simulation of Light Water Reactors (www.casl.gov), an Energy Innovation Hub (http://www.energy.gov/hubs) for Modeling and Simulation of Nuclear Reactors under US Department of Energy Contract No. DE-AC05-00OR22725. MS research is supported by the US Department of Energy, Office of Science under Contract No. DE-AC02-06CH11357. NR 33 TC 3 Z9 3 U1 1 U2 23 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 J9 J NUCL MATER JI J. Nucl. Mater. PD NOV PY 2012 VL 430 IS 1-3 BP 221 EP 228 DI 10.1016/j.jnucmat.2012.07.007 PG 8 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA 035IT UT WOS:000310940700031 ER PT J AU Wang, P Contescu, CI Yu, SY Burchell, TD AF Wang, Peng Contescu, Cristian I. Yu, Suyuan Burchell, Timothy D. TI Pore structure development in oxidized IG-110 nuclear graphite SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID OXIDATION BEHAVIOR; AIR OXIDATION; MICROSTRUCTURE; STRENGTH AB The oxidation-induced porosity development in nuclear graphite has great effect on its mechanical behavior, thus it is very important to understand the pore structure development of nuclear graphite during oxidation. This paper reports on the oxidation kinetics of grade IG-110 nuclear graphite and the porosity development in oxidized samples. The distribution of the oxidized layer in IG-110 specimens oxidized at 600-750 degrees C was studied using optical microscopy coupled with automated image analysis technique, and the mechanism of porosity development was determined. The thickness of oxidized layer decreased with the oxidation temperature but was independent of the weight loss level. Oxidation caused consumption of graphite structure and development of porosity, which was initiated from the binder phase. Statistical analysis indicated that generation and growth of pores was dominant at low temperatures, while merging and collapse of pores was the main effect at high temperatures. Compared with medium-grained PCEA graphite, the fine-grained IC-110 graphite demonstrates deeper penetration of the oxidant because of its higher pore density and greater porosity. Published by Elsevier B.V. C1 [Contescu, Cristian I.; Burchell, Timothy D.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37932 USA. [Wang, Peng; Yu, Suyuan] Tsinghua Univ, Inst Nucl & New Energy Technol, Beijing 100084, Peoples R China. RP Contescu, CI (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, 1 Bethel Valley Rd, Oak Ridge, TN 37932 USA. EM ContescuCI@ornl.gov RI Burchell, Tim/E-6566-2017; OI Burchell, Tim/0000-0003-1436-1192; Contescu, Cristian/0000-0002-7450-3722 FU United States Government [DE-AC05-00OR22725]; United States Department of Energy; US Department of Energy, Office of Nuclear Energy under NGNP Program; US Department of Energy [DE-AC05-00OR22725]; China Scholarship Council [2011621029] FX This submission was supported by a contractor of the United States Government under Contract DE-AC05-00OR22725 with the United States Department of Energy. The United States Government retains, and the publisher, by accepting this submission for publication acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this submission, or allow others to do so, for United States Government purposes.; This work was funded by the US Department of Energy, Office of Nuclear Energy under the NGNP Program. Oak Ridge National Laboratory is managed by U.T. Battelle LLC for the US Department of Energy, under Contract DE-AC05-00OR22725. P.W. acknowledges the financial support from China Scholarship Council (No. 2011621029) during his visit to Oak Ridge National Laboratory. NR 26 TC 10 Z9 10 U1 2 U2 22 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 J9 J NUCL MATER JI J. Nucl. Mater. PD NOV PY 2012 VL 430 IS 1-3 BP 229 EP 238 DI 10.1016/j.jnucmat.2012.07.015 PG 10 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA 035IT UT WOS:000310940700032 ER PT J AU Van den Berghe, S Parthoens, Y Charollais, F Kim, YS Leenaers, A Koonen, E Kuzminov, V Lemoine, P Jarousse, C Guyon, H Wachs, D Keiser, D Robinson, A Stevens, J Hofman, G AF Van den Berghe, S. Parthoens, Y. Charollais, F. Kim, Y. S. Leenaers, A. Koonen, E. Kuzminov, V. Lemoine, P. Jarousse, C. Guyon, H. Wachs, D. Keiser, D., Jr. Robinson, A. Stevens, J. Hofman, G. TI Swelling of U(Mo)-Al(Si) dispersion fuel under irradiation - Non-destructive analyses of the LEONIDAS E-FUTURE plates SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID POSTIRRADIATION EXAMINATION AB In the framework of the elimination of High-Enriched Uranium (HEU) from the civil circuit, the search for an appropriate fuel to replace the high-enriched research reactor fuel in those reactors that currently still require it for their operation has led to the development of a U-7 wt.%Mo alloy based dispersion fuel with an Al-Si matrix. The European LEONIDAS program, joining SCK center dot CEN, ILL, CEA and AREVA-CERCA, is aimed at the qualification of such a fuel for the use in high power conditions. The first experiment of the program, designated E-FUTURE, was performed to select the appropriate matrix Si concentration and fuel plate post-production heat treatment parameters for further qualification. It consisted of the irradiation of four distinct (4% and 6% Si, 3 different heat treatments) full size, flat fuel plates in the BR2 reactor. The irradiation conditions were relatively severe: 470 W/cm(2) peak BOL power, with a similar to 70% U-235 peak burnup. (C) 2012 Published by Elsevier B.V. C1 [Van den Berghe, S.; Parthoens, Y.; Leenaers, A.; Koonen, E.; Kuzminov, V.] SCK CEN, Nucl Mat Sci Inst, B-2400 Mol, Belgium. [Charollais, F.] CEA Cadarache, DEN DEC, F-13108 St Paul Les Durance, France. [Lemoine, P.] CEA Saclay, DEN DISN, F-91191 Gif Sur Yvette, France. [Jarousse, C.] AREVA CERCA, F-26104 Romans Sur Isere, France. [Guyon, H.] Inst Max Von Laue Paul Langevin, F-38042 Grenoble 9, France. [Wachs, D.; Keiser, D., Jr.; Robinson, A.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. [Kim, Y. S.; Stevens, J.; Hofman, G.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Van den Berghe, S (reprint author), SCK CEN, Nucl Mat Sci Inst, Boeretang 200, B-2400 Mol, Belgium. EM sven.van.den.berghe@sckcen.be OI Van den Berghe, Sven/0000-0002-2537-4645 NR 28 TC 18 Z9 19 U1 0 U2 14 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 J9 J NUCL MATER JI J. Nucl. Mater. PD NOV PY 2012 VL 430 IS 1-3 BP 246 EP 258 DI 10.1016/j.jnucmat.2012.06.045 PG 13 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA 035IT UT WOS:000310940700034 ER PT J AU Calzolari, A Chen, YF Lewis, GF Dougherty, DB Shultz, D Nardelli, MB AF Calzolari, Arrigo Chen, Yifeng Lewis, Geoffrey F. Dougherty, Daniel B. Shultz, David Nardelli, Marco Buongiorno TI Complex Materials for Molecular Spintronics Applications: Cobalt Bis(dioxolene) Valence Tautomers, from Molecules to Polymers SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID ORGANIC SEMICONDUCTORS; SPIN; MAGNETORESISTANCE; BISTABILITY; INJECTION; SURFACE AB Using first principles calculations, we predict a complex multifunctional behavior in cobalt bis(dioxolene) valence tautomeric compounds. Molecular spin-state switching is shown to dramatically alter electronic properties and corresponding transport properties. This spin state dependence has been demonstrated for technologically relevant coordination polymers of valence tautomers as well as for novel conjugated polymers with valence tautomeric functionalization. As a result, these materials are proposed as promising candidates for spintronic devices that can couple magnetic bistability with novel electrical and spin conduction properties. Our findings pave the way to the fundamental understanding and future design of active multifunctional organic materials for spintronics applications. C1 [Calzolari, Arrigo] CNR NANO, Ist Nanosci, I-41125 Modena, Italy. [Chen, Yifeng; Dougherty, Daniel B.] N Carolina State Univ, Dept Phys, Raleigh, NC 27695 USA. [Lewis, Geoffrey F.; Shultz, David] N Carolina State Univ, Dept Chem, Raleigh, NC 27695 USA. [Nardelli, Marco Buongiorno] Univ N Texas, Dept Phys, Denton, TX 76203 USA. [Nardelli, Marco Buongiorno] Univ N Texas, Dept Chem, Denton, TX 76203 USA. [Nardelli, Marco Buongiorno] Oak Ridge Natl Lab, CSMD, Oak Ridge, TN 37831 USA. RP Calzolari, A (reprint author), CNR NANO, Ist Nanosci, Ctr S3, I-41125 Modena, Italy. EM arrigo.calzolari@nano.cnr.it; mbn@unt.edu RI Buongiorno Nardelli, Marco/C-9089-2009; Calzolari, Arrigo/B-8448-2015 OI Calzolari, Arrigo/0000-0002-0244-7717 FU NSF-CCI Center for Molecular Spintronics [CHE-0924966]; Office of Basic Energy Sciences, U.S. Department of Energy at Oak Ridge National Laboratory [DE-AC05-00OR22725]; UT-Battelle, LLC FX This work was supported, in part, by NSF-CCI Center for Molecular Spintronics (CHE-0924966). M.B.N. wishes to acknowledge partial support from the Office of Basic Energy Sciences, U.S. Department of Energy at Oak Ridge National Laboratory under contract DE-AC05-00OR22725 with UT-Battelle, LLC. Computational resources were provided in part by NCCS-ORNL, HPC-NCSU, and CINECA (project IscraC_SHOCK). We kindly thank M. Rontani for useful discussions and a critical reading of the manuscript. NR 41 TC 15 Z9 15 U1 3 U2 47 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD NOV 1 PY 2012 VL 116 IS 43 BP 13141 EP 13148 DI 10.1021/jp3099895 PG 8 WC Chemistry, Physical SC Chemistry GA 029GM UT WOS:000310482800027 PM 23072437 ER PT J AU Kronawitter, CX Zegkinoglou, I Rogero, C Guo, JH Mao, SS Himpsel, FJ Vayssieres, L AF Kronawitter, C. X. Zegkinoglou, I. Rogero, C. Guo, J. -H. Mao, S. S. Himpsel, F. J. Vayssieres, L. TI On the Interfacial Electronic Structure Origin of Efficiency Enhancement in Hematite Photoanodes SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID RAY-ABSORPTION SPECTROSCOPY; HYDROGEN-PRODUCTION; WATER OXIDATION; THIN-FILMS; OXIDE; CELL; TIN AB The electronic structure origins of interfacial losses in hematite photoanodes and the cause of the literature-reported order-of-magnitude photocurrent increase upon short high-temperature annealing are investigated. Synchrotron-based soft X-ray absorption spectroscopy is used to probe the unoccupied states at and near the interface between hematite (alpha-Fe2O3) and fluorine-doped tin oxide (FTO). Oxygen K-edge and iron L-edge absorption spectra indicate that the interfacial interaction reduces the degree of p-d hybridization and alters the crystal field in alpha-Fe2O3. The interface is found to be associated with a distribution of unoccupied oxygen p-hybridized states located below the lowest unoccupied iron 3d states in alpha-Fe2O3 (just below the conduction band minimum), which are eliminated with high-temperature processing. These data facilitate future efforts to engineer favorable interfacial compositions and associated electrochemical potential gradients within photoanodes, which are required to efficiently separate charge carriers in operating photoelectrochemical systems such as solar cells and photocatalytic devices. C1 [Kronawitter, C. X.; Mao, S. S.] Univ Calif Berkeley, Dept Mech Engn, Berkeley, CA 94720 USA. [Kronawitter, C. X.; Mao, S. S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Zegkinoglou, I.; Himpsel, F. J.] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [Rogero, C.] Ctr Fis Mat CSIC UPV EHU, Mat Phys Ctr, San Sebastian 20018, Spain. [Zegkinoglou, I.; Guo, J. -H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Vayssieres, L.] Xi An Jiao Tong Univ, Int Res Ctr Renewable Energy, Xian 710049, Peoples R China. RP Mao, SS (reprint author), Univ Calif Berkeley, Dept Mech Engn, Berkeley, CA 94720 USA. EM ssmao@lbl.gov; fhimpsel@facstaff.wisc.edu; lionelv@xjtu.edu.cn RI Zegkinoglou, Ioannis/H-2343-2013; CSIC-UPV/EHU, CFM/F-4867-2012; OI Rogero, Celia/0000-0002-2812-8853 FU NSF/CMMI [1036076]; U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy; Office of Basic Energy Sciences [DE-SC0006931, DE-AC02-05CH11231, DE-FG02-01ER45917]; International Research Center for Renewable Energy, State Key Laboratory of Multiphase Flow in Power Engineering, Xian Jiaotong University; Thousand Talents plan; National Natural Science Foundation of China [51121092] FX This research has been supported by NSF/CMMI under grant #1036076; by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy; and by the Office of Basic Energy Sciences under the Contracts DE-SC0006931, DE-AC02-05CH11231 (ALS), DE-FG02-01ER45917 (end station). The International Research Center for Renewable Energy, State Key Laboratory of Multiphase Flow in Power Engineering, Xian Jiaotong University, the Thousand Talents plan, and the National Natural Science Foundation of China (No.51121092) are acknowledged for their support. NR 42 TC 24 Z9 24 U1 3 U2 86 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD NOV 1 PY 2012 VL 116 IS 43 BP 22780 EP 22785 DI 10.1021/jp308918e PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 029GN UT WOS:000310482900016 ER PT J AU Pollock, RA Gor, GY Walsh, BR Fry, J Ghampson, IT Melnichenko, YB Kaiser, H DeSisto, WJ Wheeler, MC Frederick, BG AF Pollock, Rachel A. Gor, Gennady Yu Walsh, Brenna R. Fry, Jason Ghampson, I. Tyrone Melnichenko, Yuri B. Kaiser, Helmut DeSisto, William J. Wheeler, M. Clayton Frederick, Brian G. TI Role of Liquid vs Vapor Water in the Hydrothermal Degradation of SBA-15 SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID ORDERED MESOPOROUS SILICAS; ANGLE NEUTRON-SCATTERING; MECHANICAL STABILITY; CATALYTIC-ACTIVITY; TRIBLOCK COPOLYMER; MOLECULAR-SIEVES; SURFACE-AREA; PORE-SIZE; MCM-41; ADSORPTION AB The hydrothermal stability of mesoporous silica is critical for applications including catalytic processing of biofuels due to the presence of significant amounts of water. We have combined neutron diffraction intensity analysis with NLDFT analysis of nitrogen sorption isotherms to characterize the spatial distribution of the secondary pore network in SBA-15 following postcalcination hydrothermal treatment in both liquid and vapor phase water at temperatures from 115 to 155 degrees C under autogenous pressure. The results are consistent with a degradation mechanism in which silica dissolves from regions of small positive curvature, e.g., near the entrance to the secondary pores, and is redeposited deeper into the framework. Pore volumes decrease fastest for the micropores and more slowly for larger secondary mesopores. Under water treatment at 115 degrees C, the mesopore diameter increases and the intrawall void fraction decreases significantly. The behavior is similar for steam treatment but occurs more slowly. Differences in the chemical environment and transport limitations are discussed. At higher temperatures of 155 degrees C, pores in the region surrounding the mesopore are nearly eliminated, trapping water deeper in the matrix, which can be seen with neutron scattering but is inaccessible to nitrogen isotherm measurements. C1 [Frederick, Brian G.] Univ Maine, LASST, Dept Chem, Orono, ME 04469 USA. [Pollock, Rachel A.] Univ Maine, Dept Phys & Astron, Orono, ME 04469 USA. [Ghampson, I. Tyrone; DeSisto, William J.; Wheeler, M. Clayton] Univ Maine, Dept Chem & Biol Engn, Lab Surface Sci & Technol, Orono, ME 04469 USA. Univ Maine, Forest Bioprod Res Inst, Orono, ME 04469 USA. [Gor, Gennady Yu] Princeton Univ, Dept Civil & Environm Engn, Princeton, NJ 08544 USA. [Fry, Jason; Kaiser, Helmut] Indiana Univ, Dept Phys, Low Energy Neutron Source, Bloomington, IN 47405 USA. [Melnichenko, Yuri B.] Oak Ridge Natl Lab, Biol & Soft Matter Div, Neutron Scattering Directorate, Oak Ridge, TN 37831 USA. [Melnichenko, Yuri B.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. RP Frederick, BG (reprint author), Univ Maine, LASST, Dept Chem, 153 ESRB Barrows Hall, Orono, ME 04469 USA. EM brian.frederick@umit.maine.edu RI Gor, Gennady/A-8090-2011; Wheeler, M Clayton/C-9649-2012 OI Gor, Gennady/0000-0001-7455-1778; Wheeler, M Clayton/0000-0003-1113-1324 FU DOE Award [DE-FG02-07ER46373]; Scientific User Facilities Division, Office of Basic Energy Science, U.S. Department of Energy FX We gratefully acknowledge support of this work through DOE Award no. DE-FG02-07ER46373. The portion of this research carried out at Oak Ridge National Laboratory's High Flux Isotope Reactor was sponsored by the Scientific User Facilities Division, Office of Basic Energy Science, U.S. Department of Energy. We also thank Roger Pynn, Carl Tripp, and Doug Ruthven for helpful discussions as well as Doug Elliott for motivating this project. NR 63 TC 15 Z9 16 U1 5 U2 47 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD NOV 1 PY 2012 VL 116 IS 43 BP 22802 EP 22814 DI 10.1021/jp303150e PG 13 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 029GN UT WOS:000310482900019 ER PT J AU Ranalli, JA Ferguson, D Martin, C AF Ranalli, Joseph A. Ferguson, Donald Martin, Christopher TI Simple Analysis of Flame Dynamics via Flexible Convected Disturbance Models SO JOURNAL OF PROPULSION AND POWER LA English DT Article ID LAMINAR PREMIXED FLAME; COMBUSTION DYNAMICS; KINEMATIC MODEL; OSCILLATIONS; PREDICTION AB Flame sheet modeling is a common approach for the determination of flame transfer functions for prediction and modeling of thermoacoustic combustion instabilities. The dynamics of the flame-sheet model for simple flame geometries can be shown to be equivalent to a basic model of convective disturbances interacting with a steady heat release region. This framework shows that the flame transfer functions predicted by linearized flame-sheet models are the Fourier transform of the steady heat release rate profile for the flamesheet geometry transformed into a Lagrangian convective time reference frame. This result is significant relative to existing flame-sheet modeling approaches in allowing the prediction of dynamic behaviors on the basis of steady information only. Multiple perturbations on the flame can be treated simply via superposition of individual perturbations. Analysis of results from these convective disturbance models illuminates the existence of two independent length scales governing the flame transfer function dynamics. Magnitude is governed by the tip-to-tail length of the flame, whereas phase is governed by the heat release rate profile center of mass calculated from the disturbance origin. The convective disturbance approach shows promise in its potential to derive flame transfer function predictions from a steady flame heat release rate profile. C1 [Martin, Christopher] Virginia Polytech & State Univ, Blacksburg, VA 24060 USA. [Ranalli, Joseph A.; Ferguson, Donald] Penn State Univ Hazleton, Natl Energy Technol Lab, Morgantown, WV 26507 USA. RP Ranalli, JA (reprint author), Penn State Univ Hazleton, Natl Energy Technol Lab, Morgantown, WV 26507 USA. EM jar339@psu.edu; donald.ferguson@netl.doe.gov; chmarti1@vt.edu FU U.S. Department of Energy; Oak Ridge Institute for Science and Education (ORISE) FX The support of the U.S. Department of Energy's Turbines program is gratefully acknowledged. Joseph A. Ranalli gratefully acknowledges the support of the Oak Ridge Institute for Science and Education (ORISE) Postdoctoral Fellowship program. NR 25 TC 0 Z9 0 U1 2 U2 5 PU AMER INST AERONAUT ASTRONAUT PI RESTON PA 1801 ALEXANDER BELL DRIVE, STE 500, RESTON, VA 22091-4344 USA SN 0748-4658 J9 J PROPUL POWER JI J. Propul. Power PD NOV-DEC PY 2012 VL 28 IS 6 BP 1268 EP 1276 DI 10.2514/1.B34405 PG 9 WC Engineering, Aerospace SC Engineering GA 037UQ UT WOS:000311132400012 ER PT J AU Vianco, P Rejent, J Grazier, M Kilgo, A AF Vianco, Paul Rejent, Jerome Grazier, Mark Kilgo, Alice TI Creep Behavior of a Sn-Ag-Bi Pb-Free Solder SO MATERIALS LA English DT Article DE tin-silver-bismuth (Sn-Ag-Bi) solder; creep deformation; aging ID TERNARY 95.5SN-3.9AG-0.6CU SOLDER; GRAIN-BOUNDARY; PART II AB Compression creep tests were performed on the ternary 91.84Sn-3.33Ag-4.83Bi (wt.%, abbreviated Sn-Ag-Bi) Pb-free alloy. The test temperatures were: -25 degrees C, 25 degrees C, 75 degrees C, 125 degrees C, and 160 degrees C (+/- 0.5 degrees C). Four loads were used at the two lowest temperatures and five at the higher temperatures. The specimens were tested in the as-fabricated condition or after having been subjected to one of two air aging conditions: 24 hours at either 125 degrees C or 150 degrees C. The strain-time curves exhibited frequent occurrences of negative creep and small-scale fluctuations, particularly at the slower strain rates, that were indicative of dynamic recrystallization (DRX) activity. The source of tertiary creep behavior at faster strain rates was likely to also be DRX rather than a damage accumulation mechanism. Overall, the strain-time curves did not display a consistent trend that could be directly attributed to the aging condition. The sinh law equation satisfactorily represented the minimum strain rate as a function of stress and temperature so as to investigate the deformation rate kinetics: d epsilon/dt(min) = Asinh(n) (alpha sigma) exp (-Delta H/RT). The values of alpha, n, and Delta H were in the following ranges (+/- 95% confidence interval): alpha, 0.010-0.015 (+/- 0.005 1/MPa); n, 2.2-3.1 (+/- 0.5); and Delta H, 54-66 (+/- 8 kJ/mol). The rate kinetics analysis indicated that short-circuit diffusion was a contributing mechanism to dislocation motion during creep. The rate kinetics analysis also determined that a minimum creep rate trend could not be developed between the as-fabricated versus aged conditions. This study showed that the elevated temperature aging treatments introduced multiple changes to the Sn-Ag-Bi microstructure that did not result in a simple loss ("softening") of its mechanical strength. C1 [Vianco, Paul; Rejent, Jerome; Grazier, Mark; Kilgo, Alice] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Vianco, P (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM ptvianc@sandia.gov; jarejen@sandia.gov; jmgrazi@sandia.gov; ackilgo@sandia.gov FU Sandia National Laboratories; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors wish to thank Don Susan for his thorough review of the manuscript. This study was supported by Sandia National Laboratories. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 22 TC 0 Z9 0 U1 2 U2 19 PU MDPI AG PI BASEL PA POSTFACH, CH-4005 BASEL, SWITZERLAND SN 1996-1944 J9 MATERIALS JI Materials PD NOV PY 2012 VL 5 IS 11 BP 2151 EP 2175 DI 10.3390/ma5112151 PG 25 WC Materials Science, Multidisciplinary SC Materials Science GA 041UI UT WOS:000311426300007 ER PT J AU Schwab, J Shen, KJ Quataert, E Dan, M Rosswog, S AF Schwab, Josiah Shen, Ken J. Quataert, Eliot Dan, Marius Rosswog, Stephan TI The viscous evolution of white dwarf merger remnants SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE hydrodynamics; supernovae: general; white dwarfs ID 3-DIMENSIONAL MAGNETOHYDRODYNAMIC SIMULATIONS; NONRADIATIVE ACCRETION FLOWS; CO-RICH MATTER; IA SUPERNOVAE; SURFACE DETONATIONS; CARBON IGNITION; MASS-TRANSFER; 2 DIMENSIONS; BLACK-HOLE; BINARIES AB The merger of two white dwarfs (WDs) creates a differentially rotating remnant which is unstable to magnetohydrodynamic instabilities. These instabilities can lead to viscous evolution on a time-scale short compared to the thermal evolution of the remnant. We present multidimensional hydrodynamic simulations of the evolution of WD merger remnants under the action of an alpha-viscosity. We initialize our calculations using the output of eight WD merger simulations from Dan et al., which span a range of mass ratios and total masses. We generically find that the merger remnants evolve towards spherical states on time-scales of hours, even though a significant fraction of the mass is initially rotationally supported. The viscous evolution unbinds only a very small amount of mass (less than or similar to 10(-5)M(circle dot)). Viscous heating causes some of the systems we study with He WD secondaries to reach conditions of nearly-dynamical burning. It is thus possible that the post-merger viscous phase triggers detonation of the He envelope in some WD mergers, potentially producing a Type Ia supernova via a double-detonation scenario. Our calculations provide the proper initial conditions for studying the long-term thermal evolution of WD merger remnants. This is important for understanding WD mergers as progenitors of Type Ia supernovae, neutron stars, R Coronae Borealis stars and other phenomena. C1 [Schwab, Josiah; Quataert, Eliot] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Schwab, Josiah; Shen, Ken J.; Quataert, Eliot] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. [Schwab, Josiah; Shen, Ken J.; Quataert, Eliot] Univ Calif Berkeley, Theoret Astrophys Ctr, Berkeley, CA 94720 USA. [Shen, Ken J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Dan, Marius; Rosswog, Stephan] Jacobs Univ Bremen, Sch Engn & Sci, D-28759 Bremen, Germany. [Rosswog, Stephan] Stockholm Univ, Dept Astron, SE-10691 Stockholm, Sweden. [Rosswog, Stephan] Stockholm Univ, Oskar Klein Ctr, SE-10691 Stockholm, Sweden. RP Schwab, J (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM jwschwab@berkeley.edu FU NSF AST [0905801]; Office of Science of the US Department of Energy [DE-AC02-05CH11231]; NSF; David and Lucile Packard Foundation; Thomas and Alison Schneider Chair in Physics; NASA [PF1-120088, NAS8-03060]; Deutsche Forschungsgemeinschaft [RO-3399/4-1, RO-3399/4-2] FX We thank Frank Timmes for making the Helmholtz EoS and the aprox13 reaction network publicly available and for a helpful email exchange related to their use. We thank Sterl Phinney, Lars Bildsten, Brian Metzger and Dan Kasen for useful conversations. JS thanks Prateek Sharma for helpful discussions about the ZEUS code. The 2D calculations were performed on Henyey, which is supported by NSF AST Grant 0905801. We thank Dan Kasen for providing computational time for our 3D calculations. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the US Department of Energy under Contract No. DE-AC02-05CH11231. JS is supported by an NSF Graduate Research Fellowship. EQ and JS are also supported in part by the David and Lucile Packard Foundation and the Thomas and Alison Schneider Chair in Physics. KJS is supported by NASA through Einstein Postdoctoral Fellowship grant number PF1-120088 awarded by the Chandra X-ray Center, which is operated by the Smithsonian Astrophysical Observatory for NASA under contract NAS8-03060. MD and SR are supported by Deutsche Forschungsgemeinschaft under grants RO-3399/4-1 and RO-3399/4-2. This research has made use of NASA's ADS Bibliographic Services. NR 50 TC 39 Z9 39 U1 0 U2 2 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0035-8711 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD NOV PY 2012 VL 427 IS 1 BP 190 EP 203 DI 10.1111/j.1365-2966.2012.21993.x PG 14 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 031XH UT WOS:000310675400016 ER PT J AU Wu, SW Liu, WT Liang, XG Schuck, PJ Wang, F Shen, YR Salmeron, M AF Wu, Shiwei Liu, Wei-Tao Liang, Xiaogan Schuck, P. James Wang, Feng Shen, Y. Ron Salmeron, Miquel TI Hot Phonon Dynamics in Graphene SO NANO LETTERS LA English DT Article DE Graphene; hot phonons; ultrafast dynamics; time resolved; anti-Stokes Raman ID SUSPENDED GRAPHENE; TRANSISTORS; DEVICES; CARBON AB The dynamics of hot phonons in supported, suspended, and gated Monolayer graphene was studied by using time-resolved anti-Stokes Raman spectroscopy. We found that the hot phonon relaxation is dominated by phonon-phonon interaction in graphene, and strongly affected by the interaction between graphene and the substrate. Relaxation via carrier-phonon coupling, known as Landau damping, is ineffective for hot phonons Which are in thermal equilibrium with excited carriers. Our findings provide a basis for better management of energy dissipation in graphene devices. C1 [Wu, Shiwei; Liang, Xiaogan; Schuck, P. James; Salmeron, Miquel] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Wang, Feng; Shen, Y. Ron; Salmeron, Miquel] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Liu, Wei-Tao; Wang, Feng; Shen, Y. Ron] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Salmeron, Miquel] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. RP Wu, SW (reprint author), Fudan Univ, Dept Phys, Shanghai 200433, Peoples R China. EM swwu@fudan.edu.cn; mbsalmeron@lbl.gov RI Wu, Shiwei/F-4542-2010; Foundry, Molecular/G-9968-2014; wang, Feng/I-5727-2015; Liu, Wei-Tao/I-9627-2014 OI Wu, Shiwei/0000-0001-9838-9066; Liu, Wei-Tao/0000-0003-0566-671X FU Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, of the U.S. Department of Energy [DE-AC02-05CH11231]; NSFC [11104036] FX This research was done at the Molecular Foundry and supported by the Director, Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, of the U.S. Department of Energy under contract no. DE-AC02-05CH11231. Manuscript finalization was also supported by NSFC under contract no. 11104036. NR 33 TC 15 Z9 15 U1 7 U2 99 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1530-6984 J9 NANO LETT JI Nano Lett. PD NOV PY 2012 VL 12 IS 11 BP 5495 EP 5499 DI 10.1021/nl301997r PG 5 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 039KJ UT WOS:000311244400009 PM 23106146 ER PT J AU Vasudevan, RK Morozovska, AN Eliseev, EA Britson, J Yang, JC Chu, YH Maksymovych, P Chen, LQ Nagarajan, V Kalinin, SV AF Vasudevan, R. K. Morozovska, A. N. Eliseev, E. A. Britson, J. Yang, J. -C. Chu, Y. -H. Maksymovych, P. Chen, L. Q. Nagarajan, V. Kalinin, S. V. TI Domain Wall Geometry Controls Conduction in Ferroelectrics SO NANO LETTERS LA English DT Article DE Domain wall conduction; PFM; phase-field modeling; c-AFM; ferroelectrics ID THIN-FILMS; BIFEO3 FILMS; POLARIZATION; MEMORY AB A new paradigm of domain wall. nanoelectronics has emerged recently, in which the domain wall in a ferroic is itself an active device element The ability to spatially. modulate the ferroic order parameter within a single domain wall allows the physical properties to be tailored at will and hence opens vastly unexplored device possibilities: Here, we demonstrate via ambient and ultrahigh-vacuum (UHV) scanning probe microscopy (SPM) measurements in bismuth ferrite that the conductivity of the domain walls can be modulated by up to 500% in the spatial dimension as a function of domain wall curvature. Landau-Ginzburg-Devonshire calculations reveal the conduction is a.. result of carriers or vacancies migrating to neutralize the charge at the farmed interface. Phase field modeling indicates that anisotropic potential distributions can occur even for initially uncharged walls, from polarization dynamics mediated by elastic effects. These results are the first proof of concept for modulation of charge as a function of domain wall geometry by a proximal probe, thereby expanding potential applications for oxide ferroics in future nanoscale electronics. C1 [Vasudevan, R. K.; Nagarajan, V.] Univ New S Wales, Sch Mat Sci & Engn, Kensington, NSW 2052, Australia. [Morozovska, A. N.] Natl Acad Sci Ukraine, Inst Phys, UA-03028 Kiev, Ukraine. [Eliseev, E. A.] Natl Acad Sci Ukraine, Inst Problems Mat Sci, UA-03028 Kiev, Ukraine. [Britson, J.; Chen, L. Q.] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. [Yang, J. -C.; Chu, Y. -H.] Natl Chiao Tung Univ, Dept Mat Sci & Engn, Hsinchu 30010, Taiwan. [Maksymovych, P.; Kalinin, S. V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Nagarajan, V (reprint author), Univ New S Wales, Sch Mat Sci & Engn, Kensington, NSW 2052, Australia. EM nagarajan@unsw.edu.au; sergei2@ornl.gov RI Ying-Hao, Chu/A-4204-2008; Chen, LongQing/I-7536-2012; Kalinin, Sergei/I-9096-2012; valanoor, nagarajan/B-4159-2012; Vasudevan, Rama/Q-2530-2015; Maksymovych, Petro/C-3922-2016 OI Ying-Hao, Chu/0000-0002-3435-9084; Chen, LongQing/0000-0003-3359-3781; Kalinin, Sergei/0000-0001-5354-6152; Vasudevan, Rama/0000-0003-4692-8579; Maksymovych, Petro/0000-0003-0822-8459 FU ARC; Australian Nanotechnology Network; NAS Ukraine; Division of Scientific User Facilities, U.S. Department of Energy; Department of Energy Basic Sciences [DOE DE-FG02-07ER46417]; National Science Council, R.O.C [NSC-101-2119-M-009-003-MY2]; Ministry of Education (MOE-ATU) [101W961]; Center for interdisciplinary science of National Chiao Tung University FX R.K.V. and V.N. acknowledge support from the ARC Discovery Project scheme and an Overseas Travel Fellowship by the Australian Nanotechnology Network. E.A.E. and A.N.M. are thankful to NAS Ukraine for support. The research at ORNL (P.M., S.V.K.) was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Division of Scientific User Facilities, U.S. Department of Energy. Computational support for this research for phase field simulations was provided by the Research Computing and Cyberinfrastructure (RCC) group, a unit of ITS at Penn State. J.B. and L.-Q.C. acknowledge funding provided by the Department of Energy Basic Sciences under Grant No. DOE DE-FG02-07ER46417. The work at National Chiao Tung University is supported by the National Science Council, R.O.C (No. NSC-101-2119-M-009-003-MY2), Ministry of Education (MOE-ATU 101W961), and Center for interdisciplinary science of National Chiao Tung University. NR 41 TC 42 Z9 42 U1 8 U2 205 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1530-6984 J9 NANO LETT JI Nano Lett. PD NOV PY 2012 VL 12 IS 11 BP 5524 EP 5531 DI 10.1021/nl302382k PG 8 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 039KJ UT WOS:000311244400014 PM 22994244 ER PT J AU Malfatti, MA Palko, HA Kuhn, EA Turteltaub, KW AF Malfatti, Michael A. Palko, Heather A. Kuhn, Edward A. Turteltaub, Kenneth W. TI Determining the Pharmacokinetics and Long-Term Biodistribution of SiO2 Nanoparticles In Vivo Using Accelerator Mass Spectrometry SO NANO LETTERS LA English DT Article DE Accelerator mass spectrometry; silica nanoparticles; pharmacokinetics; biodistribution; bioaccumulation ID MODIFIED SILICA NANOPARTICLES; QUANTUM DOTS; TISSUE DISTRIBUTION; URINARY-EXCRETION; GENE DELIVERY; DNA; CLEARANCE; BINDING; MICE; SIZE AB Biodistribution is an important factor in better. understanding silica dioxide nanoparticle (SiNP) safety. Currently, comprehensive studies on. biodistributlon are lacking, most likely due to the lack of suitable analytical methods. Accelerator mass spectrometry was used to investigate the relationship between administered dose, pharmacokinetics (PK), and long-term biodistribution of C-14-SiNPs in vivo. PK analysis showed that SiNPs were rapidly cleared from the central compartment, were distributed to tissues of the reticuloendothelial system, and persisted in the tissue over the 8 week time course, raising questions about the potential for bioaccumulation and associated long-term effects. C1 [Malfatti, Michael A.; Palko, Heather A.; Kuhn, Edward A.; Turteltaub, Kenneth W.] Lawrence Livermore Natl Lab, Biosci & Biotechnol Div, Phys & Life Sci Directorate, Livermore, CA 94550 USA. [Malfatti, Michael A.; Palko, Heather A.; Turteltaub, Kenneth W.] Battelle Ctr Fundamental & Appl Syst Toxicol B FA, Columbus, OH USA. RP Malfatti, MA (reprint author), Lawrence Livermore Natl Lab, Biosci & Biotechnol Div, Phys & Life Sci Directorate, Livermore, CA 94550 USA. FU U.S. Department of Energy by, Lawrence Livermore National Laboratory at the Research Resource for Biomedical AMS [DE-AC52-07NA27344]; National Institute of General Medical Sciences [8 P41 GM103483-14]; Battelle Memorial Institute, CRADA [PNNL/284] FX This work was performed under the auspices of the U.S. Department of Energy by, Lawrence Livermore National Laboratory at the Research Resource for Biomedical AMS under contract DE-AC52-07NA27344, and supported by grants from the National Institute of General Medical Sciences (8 P41 GM103483-14), and by Battelle Memorial Institute, CRADA No. PNNL/284. NR 43 TC 20 Z9 20 U1 1 U2 39 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1530-6984 J9 NANO LETT JI Nano Lett. PD NOV PY 2012 VL 12 IS 11 BP 5532 EP 5538 DI 10.1021/nl302412f PG 7 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 039KJ UT WOS:000311244400015 PM 23075393 ER PT J AU Dennis, AM Mangum, BD Piryatinski, A Park, YS Hannah, DC Casson, JL Williams, DJ Schaller, RD Htoon, H Hollingsworth, JA AF Dennis, Allison M. Mangum, Benjamin D. Piryatinski, Andrei Park, Young-Shin Hannah, Daniel C. Casson, Joanna L. Williams, Darrick J. Schaller, Richard D. Htoon, Han Hollingsworth, Jennifer A. TI Suppressed Blinking and Auger Recombination in Near-Infrared Type-II InP/CdS Nanocrystal Quantum Dots SO NANO LETTERS LA English DT Article DE Fluorescence blinking suppression; core/shell heterostructure; near-infrared; type-II nanocrystal quantum dot; biexciton lifetime; Auger recombination ID CDSE/CDS CORE/SHELL NANOCRYSTALS; SEMICONDUCTOR NANOCRYSTALS; SINGLE; NANOPARTICLES; FLUORESCENCE; MOLECULES; KINETICS; BEHAVIOR; AIR AB Nonblinking excitonic emission from near-infrared and type-II nanocrystal quantum dots (NQDs) is reported for the first time. To realize: this unusual degree of stability at the single-dot level, novel InP/CdS core/shell NQDs were synthesized for a range, of shell thicknesses (similar to 1-11 monolayers of CdS). Ensemble spectroscopy measurements (photoluminescence peak position And radiative lifetimes). and electronic structure calculations established the transition from type-I to type-II band alignment in these heterostructured NQDs. More significantly, single-NQD studies revealed clear evidence for blinking suppression that was not strongly shell-thickness dependent, while photobleaching and biexciton lifetimes trended explicitly with extent of shelling. Specifically, very long biexciton lifetimes-up to >7 ns-were obtained for the thickest-shell structures, indicating dramatic suppression of nonradiative Auger recombination. This new system demonstrates that electronic structure and shell thickness can be employed together to effect control over key single-dot and ensemble NQD photophysical properties. C1 [Dennis, Allison M.; Mangum, Benjamin D.; Park, Young-Shin; Williams, Darrick J.; Htoon, Han; Hollingsworth, Jennifer A.] Los Alamos Natl Lab, Mat Phys & Applicat Div, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. [Piryatinski, Andrei] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Casson, Joanna L.] Los Alamos Natl Lab, Div Chem, Los Alamos, NM 87545 USA. [Hannah, Daniel C.; Schaller, Richard D.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Schaller, Richard D.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. RP Hollingsworth, JA (reprint author), Los Alamos Natl Lab, Mat Phys & Applicat Div, Ctr Integrated Nanotechnol, POB 1663, Los Alamos, NM 87545 USA. EM jenn@lanl.gov RI Piryatinski, Andrei/B-5543-2009; OI Htoon, Han/0000-0003-3696-2896; Park, Young-Shin/0000-0003-4204-1305 FU Los Alamos National Laboratory Directed Research and Development (LDRD) Program; Single Investigator Small Group Research Grant, Office of Basic Energy Sciences (OBES), Office of Science (OS), U.S. Department of Energy (DOE) [2009LANL1096]; Center for Integrated Nanotechnologies (CINT); NIH-NIGMS [1R01GM084702-01]; National Nuclear Security Administration of the U.S. Department of Energy [DE-AC52-06NA25396]; U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX A.P. and J.C. acknowledge support by the Los Alamos National Laboratory Directed Research and Development (LDRD) Program. A.M.D., B.D.M., D.C.H. and H.H. acknowledge a Single Investigator Small Group Research Grant (2009LANL1096), Office of Basic Energy Sciences (OBES), Office of Science (OS), U.S. Department of Energy (DOE). Y.-S.P. and D.W. are supported by the Center for Integrated Nanotechnologies (CINT). J.A.H. is supported, in part, by NIH-NIGMS Grant 1R01GM084702-01. This work was performed, in part, at the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences user facility. Los Alamos National Laboratory, an affirmative action equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy under contract DE-AC52-06NA25396. Use of the Center for Nanoscale Materials (R.D.S. and D.C.H.) was supported by the U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 34 TC 59 Z9 59 U1 9 U2 136 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1530-6984 EI 1530-6992 J9 NANO LETT JI Nano Lett. PD NOV PY 2012 VL 12 IS 11 BP 5545 EP 5551 DI 10.1021/nl302453x PG 7 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 039KJ UT WOS:000311244400017 PM 23030497 ER PT J AU Tongay, S Zhou, J Ataca, C Lo, K Matthews, TS Li, JB Grossman, JC Wu, JQ AF Tongay, Sefaattin Zhou, Jian Ataca, Can Lo, Kelvin Matthews, Tyler S. Li, Jingbo Grossman, Jeffrey C. Wu, Junqiao TI Thermally Driven Crossover from Indirect toward Direct Bandgap in 2D Semiconductors: MoSe2 versus MoS2 SO NANO LETTERS LA English DT Article DE 2D-Semiconductors; MoSe2; MoS2; photoluminescence; bandgap; temperature dependence ID TRANSISTORS; PHOTOLUMINESCENCE; 2H-MOSE2; CARBON AB Layered semiconductors based on transition-metal chalcogenides usually cross from indirect bandgap in the bulk limit over to direct bandgap in the quantum (2D) limit. Such a crossover can be achieved by peeling off a multilayer sample to a single layer. For exploration of physical behavior and device applications, it is much desired to reversibly modulate such crossover in a multilayer sample. Here we demonstrate that, in a few-layer sample where the indirect bandgap and direct bandgap are nearly degenerate, the temperature rise can effectively drive the system toward the 2D limit by thermally decoupling neighboring layers via interlayer thermal expansion. Such a situation is realized in few-layer MoSe2, which shows stark contrast from the well-explored MoS2 where the indirect and direct bandgaps are far from degenerate. Photoluminescence of few-layer MoSe2 is much enhanced with the temperature rise, much like the way that the photoluminescence is enhanced due to the bandgap crossover going from the bulk to the quantum limit, offering potential applications involving external modulation of optical properties in 2D semiconductors. The direct bandgap of MoSe2, identified at 1.55 eV, may also promise applications in energy conversion involving solar spectrum, as it is close to the optimal bandgap value of single-junction solar cells and photoelechemical devices. C1 [Tongay, Sefaattin; Zhou, Jian; Lo, Kelvin; Matthews, Tyler S.; Wu, Junqiao] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Ataca, Can; Grossman, Jeffrey C.] MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA. [Li, Jingbo] Chinese Acad Sci, Inst Semicond, Beijing 100083, Peoples R China. [Wu, Junqiao] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Tongay, S (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. EM tongay@berkeley.edu; wuj@berkeley.edu RI Wu, Junqiao/G-7840-2011; Tongay, Sefaattin/E-6388-2011 OI Wu, Junqiao/0000-0002-1498-0148; FU U.S. Department of Energy [DE-FG02-11ER46796]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the U.S. Department of Energy Early Career Award DE-FG02-11ER46796. The materials preparation part was supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 33 TC 346 Z9 352 U1 46 U2 460 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1530-6984 EI 1530-6992 J9 NANO LETT JI Nano Lett. PD NOV PY 2012 VL 12 IS 11 BP 5576 EP 5580 DI 10.1021/nl302584w PG 5 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 039KJ UT WOS:000311244400022 PM 23098085 ER PT J AU Kim, J Son, H Cho, DJ Geng, BS Regan, W Shi, SF Kim, K Zettl, A Shen, YR Wang, F AF Kim, Jonghwan Son, Hyungmok Cho, David J. Geng, Baisong Regan, Will Shi, Sufei Kim, Kwanpyo Zettl, Alex Shen, Yuen-Ron Wang, Feng TI Electrical Control of Optical Plasmon Resonance with Graphene SO NANO LETTERS LA English DT Article DE Graphene; plasmon resonance; metamaterials; active plasmonics; gold nanorod; charge transfer sensor ID METAMATERIAL; MODULATOR; DYNAMICS; DEVICES; PHASE AB Surface plasmon has the unique capability to concentrate light into subwavelength volume.(1-5) Active plasmon devices using electrostatic gating can enable flexible control of the plasmon excitations,(6) which has been demonstrated recently in terahertz plasmonic structures.(7-9) Controlling plasmon resonance at optical frequencies, however, remains a significant challenge because gate-induced free, electrons have very weak responses at Optical frequencies.(10) Here we achieve :efficient control of near infrared plasmon resonance in a hybrid graphene-gold nanorod system. Exploiting the uniquely strong(11,12) and gate tunable optical transitions(13,14) of graphene, we are able to significantly modulate both the resonance. frequency and quality factor of gold nanorod plasmon. Our analysis shows that the plasmon-graphene coupling is remarkably strong: even a single electron in graphene at the plasmonic hotspot could have an observable effect on plasmon scattering intensity Such hybrid graphene-nanometallic structure provides a powerful way for electrical control of plasmon resonances at optical frequencies and could enable novel plasmonic sensing down to single charge transfer events. C1 [Kim, Jonghwan; Son, Hyungmok; Cho, David J.; Geng, Baisong; Regan, Will; Shi, Sufei; Kim, Kwanpyo; Zettl, Alex; Shen, Yuen-Ron; Wang, Feng] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Cho, David J.; Regan, Will; Kim, Kwanpyo; Zettl, Alex; Shen, Yuen-Ron; Wang, Feng] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Wang, F (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM fengwang76@berkeley.edu RI Kim, Kwanpyo/D-9121-2011; Zettl, Alex/O-4925-2016; wang, Feng/I-5727-2015; OI Kim, Kwanpyo/0000-0001-8497-2330; Zettl, Alex/0000-0001-6330-136X; Regan, William/0000-0003-0143-9827 FU Office of Basic Energy Science, Department of Energy [DE-AC02-05CH11231]; Early Career Award [DE-SC0003949]; ONR MURI [N00014-09-1-1066]; DOE Molecular Foundry [DE-AC02-05CH11231]; David and Lucile Packard fellowship FX We thank R. Segalman and B. Boudouris for providing the ionic liquid and thank X. Zhang for helpful discussion. This work was mainly supported by Office of Basic Energy Science, Department of Energy under Contract No. DE-AC02-05CH11231 Y.R.S.), and Early Career Award DE-SC0003949 (H.S. and F.W.). We also acknowledge the ONR MURI award N00014-09-1-1066 (B.G., S.S., W.R, and A.Z.), the user facility of DOE Molecular Foundry (No. DE-AC02-05CH11231), and the support from a David and Lucile Packard fellowship. F.W. designed the experiment; J.K, H.S., and D.J.C. carried out optical measurements; J.K., H.S., B.G., W.R, S.S., K.K., and A.Z. contributed to sample growth, fabrication, and characterization. J.K., Y.R.S., and F.W. performed theoretical analysis. All authors discussed the results and wrote the paper together. NR 31 TC 117 Z9 118 U1 37 U2 361 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1530-6984 J9 NANO LETT JI Nano Lett. PD NOV PY 2012 VL 12 IS 11 BP 5598 EP 5602 DI 10.1021/nl302656d PG 5 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 039KJ UT WOS:000311244400026 PM 23025816 ER PT J AU Zheng, HM Mirsaidov, UM Wang, LW Matsudaira, P AF Zheng, Haimei Mirsaidov, Utkur M. Wang, Lin-Wang Matsudaira, Paul TI Electron Beam Manipulation of Nanoparticles SO NANO LETTERS LA English DT Article DE Electron beam trap; nanoscale manipulation; liquid cell; TEM; nanoparticle interaction; directed assembly ID OPTICAL TWEEZERS; FORCES; PARTICLES; NANOCRYSTALS AB We report on electron beam: manipulation and simultaneous transmission electron microscopy imaging of gold nanoparticle movements in an environmental cell. Nanoparticles are trapped with the beam and move dynamically toward the location with higher electron density. Their global movements follow the beam positions Analysis on the trajectories of nanoparticle movements inside the beam reveals a trapping force in the piconewton range at the electron density gradient of 10(3)-10(4) (e.nm(-2).s(-1)).nm(-1). Multiple nanoparticles can also be trapped with the beam. By rapidly converging the beam, we further can "collect" nanoparticles on the membrane surface and assemble them into a cluster. C1 [Zheng, Haimei; Wang, Lin-Wang] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Mirsaidov, Utkur M.; Matsudaira, Paul] Natl Univ Singapore, MechanoBiol Inst Singapore, Singapore 117411, Singapore. [Mirsaidov, Utkur M.; Matsudaira, Paul] Natl Univ Singapore, Ctr BioImaging Sci, Dept Biol Sci, Singapore 117543, Singapore. RP Zheng, HM (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM hmzheng@lbl.gov; dbsmpt@nus.edu.sg RI Mirsaidov, Utkur/D-5821-2014; Mirsaidov, Utkur/A-6552-2012 OI Mirsaidov, Utkur/0000-0001-8673-466X; Mirsaidov, Utkur/0000-0001-8673-466X FU US DOE Office of Science Early Career Research Program FX H.Z. thanks Prof. Paul A. Alivisatos and Prof. David Chandler at the University of California, Berkeley for helpful discussions. She also thanks the support of US DOE Office of Science Early Career Research Program. NR 22 TC 27 Z9 27 U1 8 U2 86 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1530-6984 J9 NANO LETT JI Nano Lett. PD NOV PY 2012 VL 12 IS 11 BP 5644 EP 5648 DI 10.1021/nl302788g PG 5 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 039KJ UT WOS:000311244400034 PM 23035740 ER PT J AU Qadir, K Joo, SH Mun, BS Butcher, DR Renzas, JR Aksoy, F Liu, Z Somorjai, GA Park, JY AF Qadir, Kamran Joo, Sang Hoon Mun, Bongjin S. Butcher, Derek R. Renzas, J. Russell Aksoy, Funda Liu, Zhi Somorjai, Gabor A. Park, Jeong Young TI Intrinsic Relation between Catalytic Activity of CO Oxidation on Ru Nanoparticles and Ru Oxides Uncovered with Ambient Pressure XPS SO NANO LETTERS LA English DT Article DE CO oxidation; Ru nanoparticles; oxidation state; catalytic activity; nanoparticle size; ambient-pressure XPS ID RAY PHOTOELECTRON-SPECTROSCOPY; SCANNING-TUNNELING-MICROSCOPY; RUTHENIUM NANOPARTICLES; CARBON-MONOXIDE; SURFACE OXIDE; ATOMIC-SCALE; RH; RUO2(110); KINETICS; METALS AB Recent progress in colloidal synthesis of nanoparticles with well-Controlled size, shape, and composition, together with development of in situ surface science characterization tool's, such as ambient pressure X-ray photoelectron spectroscopy (APXPS), has generated new opportunities to unravel the surface structure of working catalysts. We report an APXPS study of Ru nanoparticles to investigate catalytically active species on Ru nanoparticles under oxidizing, reducing, and CO oxidation reaction conditions. The 2.8 and 6 nm Ru nanoparticle Model catalysts were synthesized in the presence of poly(vinyl pyrrolidone) polymer capping agent and deposited onto a flat Si support as two-dimensional arrays using the Langmuir-Blodgett deposition technique. Mild oxidative and reductive characteristics, indicate the formation of surface oxide on the Ru nanoparticles, the thickness of Which is found to be dependent on nanoparticle size. The larger 6 nm Ru nanoparticles were oxidized to a smaller extent than the smaller Ru 2.8 nm nanoparticles within the temperature range of 50-200 degrees C under reaction conditions, which appears to he correlated with the higher catalytic, activity of the bigger nanoparticles. We found that the smaller. Ru nanoparticle form bulk RuO2 on their. surfaces, causing the lower catalytic activity As the size of the nanoparticle. increases, the core-shell type RuO2 becomes stable. Such in situ observations of Ru nanoparticles are useful in identifying the active state of the catalysts during use and hence, may allow for rational catalyst designs for practical applications. C1 [Butcher, Derek R.; Renzas, J. Russell; Somorjai, Gabor A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Qadir, Kamran; Park, Jeong Young] Korea Adv Inst Sci & Technol, Grad Sch EEWS WCU, Taejon 305701, South Korea. [Qadir, Kamran; Park, Jeong Young] Korea Adv Inst Sci & Technol, NanoCentury KI, Taejon 305701, South Korea. [Joo, Sang Hoon] UNIST, Sch Nanobiosci & Chem Engn, KIER UNIST Adv Ctr Energy, Ulsan 689798, South Korea. [Joo, Sang Hoon] UNIST, Low Dimens Carbon Mat Ctr, Ulsan 689798, South Korea. [Mun, Bongjin S.] Hanyang Univ ERICA, Dept Appl Phys, Ansan 426791, South Korea. [Mun, Bongjin S.] Gwangju Inst Sci & Technol, Ertl Ctr Electrochem & Catalysis, Kwangju 500712, South Korea. [Aksoy, Funda; Liu, Zhi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Somorjai, GA (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM somorjai@berkeley.edu; jeongypark@kaist.ac.kr RI Joo, Sang Hoon/E-5898-2010; Mun, Bongjin /G-1701-2013; Park, Jeong Young/A-2999-2008; Liu, Zhi/B-3642-2009; Qadir, Kamran/S-8459-2016 OI Liu, Zhi/0000-0002-8973-6561; Qadir, Kamran/0000-0002-0378-2488 FU Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering of the U.S. Department of Energy [DE-AC02-05CH11231]; WCU (World Class University) program [31-2008-000-10055-0]; National Research Foundation [KRF-2012-009249]; Fundamental R&D Program for Core Technology of Materials; Ministry of Knowledge Economy, Republic of Korea; Basic Science Research Program through the National Research Foundation of Korea; Ministry of Education, Science and Technology [2012-0003813]; TJ Park Junior Faculty Fellowship FX This work was supported by the Director, Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231, and partly by WCU (World Class University) program (31-2008-000-10055-0) and KRF-2012-009249 through the National Research Foundation and from the Fundamental R&D Program for Core Technology of Materials funded by the Ministry of Knowledge Economy, Republic of Korea. S.H.J. was supported by the Basic Science Research Program through the National Research Foundation of Korea funded by the Ministry of Education, Science and Technology (2012-0003813) and by TJ Park Junior Faculty Fellowship. NR 46 TC 59 Z9 59 U1 6 U2 171 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1530-6984 J9 NANO LETT JI Nano Lett. PD NOV PY 2012 VL 12 IS 11 BP 5761 EP 5768 DI 10.1021/nl303072d PG 8 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 039KJ UT WOS:000311244400054 PM 23067327 ER PT J AU Hassoun, J Jung, HG Lee, DJ Park, JB Amine, K Sun, YK Scrosati, B AF Hassoun, Jusef Jung, Hun-Gi Lee, Dong-Ju Park, Jin-Bum Amine, Khalil Sun, Yang-Kook Scrosati, Bruno TI A Metal-Free, Lithium-Ion Oxygen Battery: A Step Forward to Safety in Lithium-Air Batteries SO NANO LETTERS LA English DT Article DE Lithium-ion oxygen cell; lithiated silicon-carbon anode; reversible charge-discharge process; rechargeable lithium metal-free-air battery ID ELECTROLYTES; ENERGY AB A preliminary study of the behavior of lithium-ion-air battery, where the common, unsafe lithium metal anode is replaced by a lithiated silicon-carbon composite, is reported. The results based on X-ray diffraction and galvanostatic charge-discharge analyses, demonstrate, the basic reversibility of the electrochemical process of the battery that can be promisingly cycled with a rather high specific capacity. C1 [Hassoun, Jusef; Scrosati, Bruno] Univ Roma La Sapienza, Dept Chem, I-00185 Rome, Italy. [Jung, Hun-Gi; Lee, Dong-Ju; Park, Jin-Bum; Sun, Yang-Kook] Hanyang Univ, Dept WCU Energy Engn, Seoul 133791, South Korea. [Amine, Khalil] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Hassoun, J (reprint author), Univ Roma La Sapienza, Dept Chem, I-00185 Rome, Italy. EM jusef.hassoun@uniroma1.it; yksun@hanyang.ac.kr; bruno.scrosati@uniroma1.it RI Sun, Yang-Kook/B-9157-2013; Amine, Khalil/K-9344-2013; Jung, Hun-Gi/P-8305-2014; OI Sun, Yang-Kook/0000-0002-0117-0170; Hassoun, Jusef/0000-0002-8218-5680 FU Human Resources Development of the Korea Institute of Energy Technology Evaluation and Planning (KETEP); Korea government Ministry of Knowledge Economy [20114010203150]; Project "REALIST"(Rechargeable, advanced, nano structured lithium batteries with high energy storage); Italian Institute of Technology (IIT) FX This work was supported by the Human Resources Development of the Korea Institute of Energy Technology Evaluation and Planning (KETEP) grant funded by the Korea government Ministry of Knowledge Economy (No. 20114010203150) and by the Project "REALIST"(Rechargeable, advanced, nano structured lithium batteries with high energy storage) sponsored by Italian Institute of Technology (IIT). This work has been performed in collaboration with Argonne National laboratory. The authors wish to thank Professor Sung-Man Lee of Kangwon National University, South Korea for kindly supplying the silicon-C electrode. NR 25 TC 68 Z9 69 U1 18 U2 212 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1530-6984 J9 NANO LETT JI Nano Lett. PD NOV PY 2012 VL 12 IS 11 BP 5775 EP 5779 DI 10.1021/nl303087j PG 5 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 039KJ UT WOS:000311244400056 PM 23077970 ER PT J AU Hannah, DC Ithurria, S Krylova, G Talapin, DV Schatz, GC Schaller, RD AF Hannah, Daniel C. Ithurria, Sandrine Krylova, Galyna Talapin, Dmitri V. Schatz, George C. Schaller, Richard D. TI Particle-Level Engineering of Thermal Conductivity in Matrix-Embedded Semiconductor Nanocrystals SO NANO LETTERS LA English DT Article DE Quantum dot; phonon; thermal transport; semiconductor; spectroscopy ID QUANTUM DOTS; AQUEOUS-SOLUTION; RELAXATION; NANOPARTICLES; CDSE; PROBES AB Known manipulations of semiconductor thermal transport properties rely upon higher-order material organization. Here, using time-resolved optical signatures of phonon transport, we demonstrate a "bottom-up" means of controlling thermal outflow in matrix embedded semiconductor nanocrystals. Growth of an electronically noninteracting ZnS shell on a CdSe core modifies thermalization times by an amount proportional to the overall particle radius. Using this approach, we obtain changes in effective thermal conductivity of up to 5x for a nearly constant energy gap. C1 [Hannah, Daniel C.; Schatz, George C.; Schaller, Richard D.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Ithurria, Sandrine; Talapin, Dmitri V.] Univ Chicago, Dept Chem, Chicago, IL 60637 USA. [Ithurria, Sandrine; Talapin, Dmitri V.] Univ Chicago, James Franck Inst, Chicago, IL 60637 USA. [Krylova, Galyna; Talapin, Dmitri V.; Schaller, Richard D.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. RP Schaller, RD (reprint author), Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. EM schaller@anl.gov FU Center for Nanoscale Materials, a U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility [DE-AC02-06CH11357]; Office of Basic Energy Sciences, U.S. Department of Energy [DE-SC0004752]; NSF [DGE-0824162]; University of Chicago; Department of Energy [DE-AC02-06CH11357] FX This work was performed, in part, at the Center for Nanoscale Materials, a U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility under Contract No. DE-AC02-06CH11357. D.C.H. and G.C.S. were supported by Grant DE-SC0004752 of the Office of Basic Energy Sciences, U.S. Department of Energy. D.C.H. acknowledges support from NSF Graduate Fellowship DGE-0824162. S.I., D.V.T., and R.D.S. acknowledge support from the University of Chicago and the Department of Energy under Contract No. DE-AC02-06CH11357 awarded to UChicago Argonne, LLC, operator of Argonne National Laboratory. NR 30 TC 2 Z9 2 U1 1 U2 46 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1530-6984 J9 NANO LETT JI Nano Lett. PD NOV PY 2012 VL 12 IS 11 BP 5797 EP 5801 DI 10.1021/nl303109r PG 5 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 039KJ UT WOS:000311244400060 PM 23066718 ER PT J AU Le, ST Jannaty, P Luo, X Zaslavsky, A Perea, DE Dayeh, SA Picraux, ST AF Le, Son T. Jannaty, P. Luo, Xu Zaslavsky, A. Perea, Daniel E. Dayeh, Shadi A. Picraux, S. T. TI Axial SiGe Heteronanowire Tunneling Field-Effect Transistors SO NANO LETTERS LA English DT Article DE SiGe heteronanowire; tunneling field effect transistor; axial heterojunction; VLS growth ID GERMANIUM NANOWIRES; SILICON; GROWTH AB We present silicon-compatible trigated p-Ge/i-Si/n-Si axial heteronanowire tunneling field-effect transistors (TFETs), where on-state tunneling occurs in the Ge drain section, while off-state leakage is dominated by the Si junction in the source. Our TFETs have high I-ON similar to 2 mu A/mu m, fully suppressed ambipolarity, and a subthreshold slope SS similar to 140 mV/decade over 4 decades of current with lowest SS similar to 50 mV/decade. Device operation in the tunneling mode is confirmed by three-dimensional TCAD simulation. Interestingly, in addition to the TFET mode, our devices work as standard nanowire FETs with a good I-ON/I-OFF ratio when the source-drain junction is forward-biased. The improved transport in both biasing modes confirms the benefits of utilizing bandgap engineered axial nanowires for enhancing device performance. C1 [Le, Son T.; Jannaty, P.; Luo, Xu; Zaslavsky, A.] Brown Univ, Dept Phys, Providence, RI 02912 USA. [Le, Son T.; Jannaty, P.; Luo, Xu; Zaslavsky, A.] Brown Univ, Sch Engn, Providence, RI 02912 USA. [Perea, Daniel E.] Pacific NW Natl Lab, Environm & Mol Sci Lab, Richland, WA 99352 USA. [Dayeh, Shadi A.; Picraux, S. T.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. [Dayeh, Shadi A.] Univ Calif San Diego, Dept Elect & Comp Engn, La Jolla, CA 92093 USA. RP Le, ST (reprint author), Brown Univ, Dept Phys, Providence, RI 02912 USA. EM son_le@brown.edu; alexander_zaslavsky@brown.edu RI Zaslavsky, Alexander/F-6232-2012; Perea, Daniel/A-5345-2010 FU NSF [ECCS-1068895, DMR-1203186]; Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences user facility at Los Alamos National Laboratory [DE-AC52-06NA25396]; Sandia National Laboratories [DE-AC04-94AL85000]; LANL LDRD program; Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory FX The work at Brown was supported by the NSF (awards ECCS-1068895 and DMR-1203186). Heteronanowire epitaxy was performed at the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences user facility at Los Alamos National Laboratory (Contract DE-AC52-06NA25396) and Sandia National Laboratories (Contract DE-AC04-94AL85000), and the work was supported in part by the LANL LDRD program. A portion of the research was performed using EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. The authors would like to thank Brown's Center for Computation and Visualization for making the Oscar cluster available for device simulations. We would like to thank Dr. Aditya Mohite, CINT-LANL for useful discussions and advises on device fabrication throughout the project. NR 31 TC 21 Z9 21 U1 1 U2 54 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1530-6984 J9 NANO LETT JI Nano Lett. PD NOV PY 2012 VL 12 IS 11 BP 5850 EP 5855 DI 10.1021/nl3032058 PG 6 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 039KJ UT WOS:000311244400070 PM 23113718 ER PT J AU Kim, BJ Wen, CY Tersoff, J Reuter, MC Stach, EA Ross, FM AF Kim, B. J. Wen, C. -Y. Tersoff, J. Reuter, M. C. Stach, E. A. Ross, F. M. TI Growth Pathways in Ultralow Temperature Ge Nucleation from Au SO NANO LETTERS LA English DT Article DE Catalytic growth; chemical vapor deposition; germanium; low temperature growth; vapor-liquid-solid growth; vapor-solid-solid growth ID GERMANIUM NANOWIRES; SILICON NANOWIRES; EUTECTIC TEMPERATURE; ORIENTATION; CATALYSTS; WHISKERS; EPITAXY AB Device integration on flexible or low-cost substrates, hag, driven, interest in the low-temperature,growth of semiconduct nanostructures. Using in situ electron microscopy, we examine the Au catalyzed growth of crystalline Ge at temperatures as low as 150 degrees C. For this materials system, the model for low temperature growth of nanowires, we find three distinct reaction pathways The lowest temperature reactions are distinguished by the absence of any purely liquid state. From measurements of reaction rates and parameters such as super saturation, we explain the sequence of pathways as arising from a kinetic competition between the imposed time scale for Ge addition and the inherent time scale for Ge nucleation. This enables an understanding of the conditions tinder which catalytic Ge growth can occur at very low temperatures, with implications for nanostructure formation on temperature sensitive substrates. C1 [Wen, C. -Y.; Stach, E. A.] Purdue Univ, Birck Nanotechnol Ctr, W Lafayette, IN 47907 USA. [Tersoff, J.; Reuter, M. C.; Ross, F. M.] IBM TJ Watson Res Ctr, Yorktown Hts, NY USA. [Stach, E. A.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Kim, B. J.] Gwangju Inst Sci & Technol, Dept Mat Sci & Engn, Kwangju, South Korea. RP Stach, EA (reprint author), Purdue Univ, Birck Nanotechnol Ctr, W Lafayette, IN 47907 USA. EM estach@bnl.gov; fmross@us.ibm.com RI Stach, Eric/D-8545-2011 OI Stach, Eric/0000-0002-3366-2153 FU NSF [DMR-0606395, DMR-0907483]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX The authors acknowledge financial assistance from the NSF under Grants No. DMR-0606395 and DMR-0907483. Research was carried out in part at the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. We gratefully acknowledge the help of Andrew D. Gamalski in calculating the thermodynamics of the Au-Ge system. NR 32 TC 15 Z9 15 U1 1 U2 66 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1530-6984 J9 NANO LETT JI Nano Lett. PD NOV PY 2012 VL 12 IS 11 BP 5867 EP 5872 DI 10.1021/nl303225a PG 6 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 039KJ UT WOS:000311244400073 PM 23121486 ER PT J AU Wang, JW Liu, XH Mao, SX Huang, JY AF Wang, Jiang Wei Liu, Xiao Hua Mao, Scott X. Huang, Jian Yu TI Microstructural Evolution of Tin Nanoparticles during In Situ Sodium Insertion and Extraction SO NANO LETTERS LA English DT Article DE Tin nanoparticles; sodiation; amorphous NaxSn alloy; Na15Sn4; sodium ion battery; in situ transmission electron microscopy ID TRANSMISSION ELECTRON-MICROSCOPY; LITHIUM ION BATTERIES; ELECTROCHEMICAL LITHIATION; SILICON NANOWIRES; ANODES; DELITHIATION; CHALLENGES; FRACTURE; STORAGE; CARBON AB The microstructural changes and phase transformations of tin nanoparticles during electrochemical sodiation were studied with a nanosized sodium ion battery using in situ transmission electron microscopy. It was found that the first sodiation process occurred in two steps; that is, the crystalline Sn nanoparticles were initially sodiated via a two-phase mechanism with a migrating phase boundary to form a Na-poor, amorphous NaxSn alloy (x similar to 0.5), which was further sodiated to several Na-rich amorphous phases and finally to the crystallized Na15Sn4 (x = 3.75) via a single-phase mechanism. The volumetric expansion was about 60% in the first step and 420% after the second step. However, despite the huge expansion, cracking or fracture was not observed, which is attributed to the second step of the single-phase sodiation that accommodates large portion of the sodiation-induced stress over the entire particle. Excellent cyclability was also observed during the reversible sodiation/desodiation cycles, showing great potential of Sn nanoparticles as a robust electrode material for rechargeable batteries. C1 [Liu, Xiao Hua; Huang, Jian Yu] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA. [Wang, Jiang Wei; Mao, Scott X.] Univ Pittsburgh, Dept Mech Engn & Mat Sci, Pittsburgh, PA 15261 USA. RP Liu, XH (reprint author), Sandia Natl Labs, Ctr Integrated Nanotechnol, POB 5800, Albuquerque, NM 87185 USA. EM lxhua99@gmail.com; sxm2@pitt.edu; jyhuang8@yahoo.com RI Wang, Jiangwei/F-8249-2011; Liu, Xiaohua/A-8752-2011 OI Wang, Jiangwei/0000-0003-1191-0782; Liu, Xiaohua/0000-0002-7300-7145 FU Laboratory Directed Research and Development (LDRD) project at Sandia National Laboratories (SNL); Nanostructures for Electrical Energy Storage (NEES), an Energy Frontier Research Center (EFRC); U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DESC0001160]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; NSF CMMI through University of Pittsburgh [08 010934] FX Portions of this work were supported by a Laboratory Directed Research and Development (LDRD) project at Sandia National Laboratories (SNL) and partly by Nanostructures for Electrical Energy Storage (NEES), an Energy Frontier Research Center (EFRC) funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award No. DESC0001160. The LDRD supported the development and fabrication of platforms. The NEES center supported the development of TEM techniques. The Sandia-Los Alamos Center for Integrated Nanotechnologies (CINT) supported the TEM capability. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Company, for the U.S. Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL85000. S.X.M. acknowledges NSF CMMI 08 010934 through University of Pittsburgh and Sandia National Lab support. NR 37 TC 164 Z9 169 U1 29 U2 344 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1530-6984 J9 NANO LETT JI Nano Lett. PD NOV PY 2012 VL 12 IS 11 BP 5897 EP 5902 DI 10.1021/nl303305c PG 6 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA 039KJ UT WOS:000311244400078 PM 23092238 ER PT J AU Iyer, S Doktycz, MJ AF Iyer, Sukanya Doktycz, Mitchel J. TI Shear-activated nanotherapeutics SO NANOMEDICINE LA English DT News Item C1 [Iyer, Sukanya; Doktycz, Mitchel J.] Univ Tennessee, Grad Program Genome Sci & Technol, Knoxville, TN 37996 USA. [Iyer, Sukanya; Doktycz, Mitchel J.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. [Doktycz, Mitchel J.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Doktycz, MJ (reprint author), Univ Tennessee, Grad Program Genome Sci & Technol, Knoxville, TN 37996 USA. EM doktyczmj@ornl.gov RI Doktycz, Mitchel/A-7499-2011 OI Doktycz, Mitchel/0000-0003-4856-8343 NR 0 TC 1 Z9 1 U1 1 U2 11 PU FUTURE MEDICINE LTD PI LONDON PA UNITEC HOUSE, 3RD FLOOR, 2 ALBERT PLACE, FINCHLEY CENTRAL, LONDON, N3 1QB, ENGLAND SN 1743-5889 J9 NANOMEDICINE-UK JI Nanomedicine PD NOV PY 2012 VL 7 IS 11 BP 1653 EP 1653 PG 1 WC Biotechnology & Applied Microbiology; Nanoscience & Nanotechnology SC Biotechnology & Applied Microbiology; Science & Technology - Other Topics GA 040NN UT WOS:000311329700007 PM 23210713 ER PT J AU Whitney, JR Rodgers, A Harvie, E Carswell, WF Torti, S Puretzky, AA Rouleau, CM Geohegan, DB Rylander, CG Rylander, MN AF Whitney, Jon R. Rodgers, Amanda Harvie, Erica Carswell, William F. Torti, Suzy Puretzky, Alex A. Rouleau, Christoper M. Geohegan, David B. Rylander, Christoper G. Rylander, Marissa N. TI Spatial and temporal measurements of temperature and cell viability in response to nanoparticle-mediated photothermal therapy SO NANOMEDICINE LA English DT Article DE cancer; carbon nanohorn; photothermal; spatiotemporal viability ID WALLED CARBON NANOHORNS; HUMAN NEUROBLASTOMA-CELLS; NATURAL-CONVECTION PLUME; CANCER; HYPERTHERMIA; NANOTUBES; APOPTOSIS; DESTRUCTION; TOXICITY; ABLATION AB Aim: Nanoparticle-enhanced photothermal therapy is a promising alternative to tumor resection. However, quantitative measurements of cellular response to these treatments are limited. This article introduces a Bimodal Enhanced Analysis of Spatiotemporal Temperature (BEAST) algorithm to rapidly determine the viability of cancer cells in vitro following photothermal therapy alone or in combination with nanoparticles. Materials & methods: To illustrate the capability of the BEAST viability algorithm, single wall carbon nanohorns were added to renal cancer (RENCA) cells in vitro and time-dependent spatial temperature maps measured with an infrared camera during laser therapy were correlated with post-treatment cell viability distribution maps obtained by cell-staining fluorescent microscopy. Conclusion: The BEAST viability algorithm accurately and rapidly determined the cell viability as a function of time, space and temperature. C1 [Whitney, Jon R.; Harvie, Erica; Rylander, Christoper G.; Rylander, Marissa N.] Virginia Tech, Dept Mech Engn, Blacksburg, VA 24061 USA. [Whitney, Jon R.; Harvie, Erica; Rylander, Christoper G.; Rylander, Marissa N.] Virginia Tech, Sch Biomed Engn & Sci, Blacksburg, VA 24061 USA. [Rodgers, Amanda] Virginia Tech, Dept Ind Syst & Engn, Blacksburg, VA 24061 USA. [Carswell, William F.] Virginia Tech, Dept Biol Syst Engn, Blacksburg, VA 24061 USA. [Torti, Suzy] Univ Connecticut, Farmington, CT 06030 USA. [Puretzky, Alex A.; Rouleau, Christoper M.; Geohegan, David B.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Whitney, JR (reprint author), ICTAS 410 ICTAS, Stanger St,MC 0193, Blacksburg, VA 24061 USA. EM jonwhit@vt.edu RI Geohegan, David/D-3599-2013; Rylander, Chris /F-2454-2014; Rylander, Marissa Nichole/F-2455-2014; Rouleau, Christopher/Q-2737-2015; Puretzky, Alexander/B-5567-2016 OI Geohegan, David/0000-0003-0273-3139; Rouleau, Christopher/0000-0002-5488-3537; Puretzky, Alexander/0000-0002-9996-4429 FU National Science Foundation [0731108, 0933571, 0955072]; NIH [1 R21 CA135230-01, R21 CA 156078, RO1CA128428]; Institute for Critical Technology and Applied Science (ICTAS, Virginia Tech, VA, USA); Office of Basic Energy Sciences, US Department of Energy; Materials Sciences and Engineering Division, Office of Basic Energy Sciences, US Department of Energy FX Funding was provided by the National Science Foundation Grants 0731108, 0933571 and 0955072, NIH Grants 1 R21 CA135230-01, R21 CA 156078 and RO1CA128428, and an Institute for Critical Technology and Applied Science (ICTAS, Virginia Tech, VA, USA) Grant. A portion of this research was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Office of Basic Energy Sciences, US Department of Energy. Single-walled carbon nanohorns were synthesized under research sponsored by the Materials Sciences and Engineering Division, Office of Basic Energy Sciences, US Department of Energy. Materials synthesized under research sponsored by the Materials Sciences and Engineering Division, Office of Basic Energy Sciences, US Department of Energy. The authors have no other relevant affiliations or financial involvement with any organization or entity with a financial interest in or financial conflict with the subject matter or materials discussed in the manuscript apart from those disclosed. NR 45 TC 8 Z9 9 U1 0 U2 23 PU FUTURE MEDICINE LTD PI LONDON PA UNITEC HOUSE, 3RD FLOOR, 2 ALBERT PLACE, FINCHLEY CENTRAL, LONDON, N3 1QB, ENGLAND SN 1743-5889 EI 1748-6963 J9 NANOMEDICINE-UK JI Nanomedicine PD NOV PY 2012 VL 7 IS 11 BP 1729 EP 1742 DI 10.2217/NNM.12.66 PG 14 WC Biotechnology & Applied Microbiology; Nanoscience & Nanotechnology SC Biotechnology & Applied Microbiology; Science & Technology - Other Topics GA 040NN UT WOS:000311329700016 PM 22812710 ER PT J AU Lou, CB Stanton, B Chen, YJ Munsky, B Voigt, CA AF Lou, Chunbo Stanton, Brynne Chen, Ying-Ja Munsky, Brian Voigt, Christopher A. TI Ribozyme-based insulator parts buffer synthetic circuits from genetic context SO NATURE BIOTECHNOLOGY LA English DT Article ID ESCHERICHIA-COLI; NOISE-PROPAGATION; SELF-CLEAVAGE; BIOLOGY; RNA; CONSTRUCTION; SATELLITE; SEQUENCE; EXPRESSION; NETWORKS AB Synthetic genetic programs are built from circuits that integrate sensors and implement temporal control of gene expression(1-4). Transcriptional circuits are layered by using promoters to carry the signal between circuits. In other words, the output promoter of one circuit serves as the input promoter to the next. Thus, connecting circuits requires physically connecting a promoter to the next circuit. We show that the sequence at the junction between the input promoter and circuit can affect the input-output response (transfer function) of the circuit(5-9). A library of putative sequences that might reduce (or buffer) such context effects, which we refer to as 'insulator parts', is screened in Escherichia coli. We find that ribozymes that cleave the 5' untranslated region (5'-UTR) of the mRNA are effective insulators. They generate quantitatively identical transfer functions, irrespective of the identity of the input promoter. When these insulators are used to join synthetic gene circuits, the behavior of layered circuits can be predicted using a mathematical model. The inclusion of insulators will be critical in reliably permuting circuits to build different programs. C1 [Lou, Chunbo; Stanton, Brynne; Chen, Ying-Ja; Voigt, Christopher A.] MIT, Dept Biol Engn, Synthet Biol Ctr, Cambridge, MA 02139 USA. [Munsky, Brian] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM USA. [Munsky, Brian] Los Alamos Natl Lab, Comp Computat & Stat Sci Div, Los Alamos, NM USA. RP Voigt, CA (reprint author), MIT, Dept Biol Engn, Synthet Biol Ctr, 77 Massachusetts Ave, Cambridge, MA 02139 USA. EM cavoigt@gmail.com RI Munsky, Brian/A-1947-2016 OI Munsky, Brian/0000-0001-6147-7329 FU Defense Advanced Research Projects Agency Chronicle of Lineage Indicative of Origins (DARPA CLIO) [N66001-12-C-4018]; Office of Naval Research [N00014-10-1-0245]; National Science Foundation (NSF) [CCF-0943385]; National Institutes of Health [AI067699]; NSF Synthetic Biology Engineering Research Center (SynBERC) [SA5284-11210]; Life Technologies FX C.A.V. is supported by Life Technologies, Defense Advanced Research Projects Agency Chronicle of Lineage Indicative of Origins (DARPA CLIO, N66001-12-C-4018), Office of Naval Research (N00014-10-1-0245), National Science Foundation (NSF) (CCF-0943385), National Institutes of Health (AI067699) and the NSF Synthetic Biology Engineering Research Center (SynBERC, SA5284-11210). NR 48 TC 98 Z9 99 U1 3 U2 61 PU NATURE PUBLISHING GROUP PI NEW YORK PA 75 VARICK ST, 9TH FLR, NEW YORK, NY 10013-1917 USA SN 1087-0156 J9 NAT BIOTECHNOL JI Nat. Biotechnol. PD NOV PY 2012 VL 30 IS 11 BP 1137 EP + DI 10.1038/nbt.2401 PG 7 WC Biotechnology & Applied Microbiology SC Biotechnology & Applied Microbiology GA 037FL UT WOS:000311087500034 PM 23034349 ER PT J AU Cheng, PN Liu, C Zhao, ML Eisenberg, D Nowick, JS AF Cheng, Pin-Nan Liu, Cong Zhao, Minglei Eisenberg, David Nowick, James S. TI Amyloid beta-sheet mimics that antagonize protein aggregation and reduce amyloid toxicity SO NATURE CHEMISTRY LA English DT Article ID SOLID-STATE NMR; A-BETA; ALZHEIMERS-DISEASE; FIBRILS; OLIGOMERIZATION; ORGANIZATION; POLYMORPHISM; MUTATIONS; PEPTIDES; REVEAL AB The amyloid protein aggregation associated with diseases such as Alzheimer's, Parkinson's and type II diabetes (among many others) features a bewildering variety of beta-sheet-rich structures in transition from native proteins to ordered oligomers and fibres. The variation in the amino-acid sequences of the beta-structures presents a challenge to developing a model system of beta-sheets for the study of various amyloid aggregates. Here, we introduce a family of robust beta-sheet macrocycles that can serve as a platform to display a variety of heptapeptide sequences from different amyloid proteins. We have tailored these amyloid beta-sheet mimics (ABSMs) to antagonize the aggregation of various amyloid proteins, thereby reducing the toxicity of amyloid aggregates. We describe the structures and inhibitory properties of ABSMs containing amyloidogenic peptides from the amyloid-beta peptide associated with Alzheimer's disease, beta(2)-microglobulin associated with dialysis-related amyloidosis, alpha-synuclein associated with Parkinson's disease, islet amyloid polypeptide associated with type II diabetes, human and yeast prion proteins, and Tau, which forms neurofibrillary tangles. C1 [Cheng, Pin-Nan; Nowick, James S.] Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA. [Liu, Cong; Zhao, Minglei; Eisenberg, David] Univ Calif Los Angeles, Howard Hughes Med Inst, Inst Mol Biol, UCLA DOE Inst Genom & Prote, Los Angeles, CA 90095 USA. RP Cheng, PN (reprint author), Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA. EM david@mbi.ucla.edu; jsnowick@uci.edu RI Zhao, Minglei/J-4446-2015 OI Zhao, Minglei/0000-0001-5832-6060 FU NIH [5R01 GM049076, 1R01 GM097562, 1R01 AG029430]; NSF [CHE-1112188, CHE-0750523, MCB-0445429]; HHMI FX The authors acknowledge support from the NIH (5R01 GM049076, 1R01 GM097562 and 1R01 AG029430), the NSF (CHE-1112188, CHE-0750523 and MCB-0445429) and HHMI. The authors also thank A. Berk and D. Gou for help with tissue culture experiments, and S. Blum for suggestions for Fig. 5a. NR 36 TC 81 Z9 83 U1 11 U2 124 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1755-4330 J9 NAT CHEM JI Nat. Chem. PD NOV PY 2012 VL 4 IS 11 BP 927 EP 933 DI 10.1038/NCHEM.1433 PG 7 WC Chemistry, Multidisciplinary SC Chemistry GA 028QG UT WOS:000310436600012 PM 23089868 ER PT J AU Gross, E Liu, JHC Toste, FD Somorjai, GA AF Gross, Elad Liu, Jack Hung-Chang Toste, F. Dean Somorjai, Gabor A. TI Control of selectivity in heterogeneous catalysis by tuning nanoparticle properties and reactor residence time SO NATURE CHEMISTRY LA English DT Article ID SURFACE ORGANOMETALLIC CHEMISTRY; GOLD NANOPARTICLES; METAL NANOPARTICLES; COUPLING REACTIONS; MESOPOROUS SILICA; FACILE SYNTHESIS; ALKYNES; ALUMINA AB A combination of the advantages of homogeneous and heterogeneous catalysis could enable the development of sustainable catalysts with novel reactivity and selectivity. Although heterogeneous catalysts are often recycled more easily than their homogeneous counterparts, they can be difficult to apply in traditional organic reactions and modification of their properties towards a desired reactivity is, at best, complex. In contrast, tuning the properties of homogeneous catalysts by, for example, modifying the ligands that coordinate a metal centre is better understood. Here, using olefin cyclopropanation reactions catalysed by dendrimer-encapsulated Au nanoclusters as examples, we demonstrate that changing the dendrimer properties allows the catalytic reactivity to be tuned in a similar fashion to ligand modification in a homogeneous catalyst. Furthermore, we show that these heterogeneous catalysts employed in a fixed-bed flow reactor allow fine control over the residence time of the reactants and thus enables the control over product distribution in a way that is not easily available for homogeneous catalysts. C1 [Gross, Elad] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. RP Gross, E (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. EM fdtoste@berkeley.edu; somorjai@berkeley.edu RI Foundry, Molecular/G-9968-2014; OI Toste, F. Dean/0000-0001-8018-2198 FU Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geological and Biosciences of the US Department of Energy (DOE) [DE-AC02-05CH11231]; Office of Science, Office of Basic Energy Sciences of the US DOE [DE-AC02-05CH11231] FX We acknowledge support from the Director, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geological and Biosciences of the US Department of Energy (DOE) under contract DE-AC02-05CH11231. Nanoparticle TEM imaging was performed by S. Alayoglu at the Molecular Foundry Imaging Facility, Lawrence Berkeley National Laboratory, which is supported by the Office of Science, Office of Basic Energy Sciences of the US DOE under contract DE-AC02-05CH11231. NR 35 TC 99 Z9 100 U1 18 U2 250 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1755-4330 J9 NAT CHEM JI Nat. Chem. PD NOV PY 2012 VL 4 IS 11 BP 947 EP 952 DI 10.1038/NCHEM.1465 PG 6 WC Chemistry, Multidisciplinary SC Chemistry GA 028QG UT WOS:000310436600015 PM 23089871 ER PT J AU Thome, L Moll, S Debelle, A Garrido, F Sattonnay, G Jagielski, J AF Thome, L. Moll, S. Debelle, A. Garrido, F. Sattonnay, G. Jagielski, J. TI Use of channeling for the study of radiation effects in nuclear materials SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS LA English DT Article; Proceedings Paper CT 20th International Conference on Ion Beam Analysis (IBA) CY APR 10-15, 2011 CL Univ Fed Rio Grande Sul (UFRGS), Inst Phys, Ion Implantat Lab, Itapema, BRAZIL HO Univ Fed Rio Grande Sul (UFRGS), Inst Phys, Ion Implantat Lab DE Nuclear materials; Ion irradiation; SHIBIEC ID HEAVY-ION IRRADIATION; SINGLE-CRYSTALS; QUANTITATIVE-ANALYSIS; PYROCHLORE OXIDES; DAMAGE EVOLUTION; CERAMICS; ZIRCONIA; SPINEL; WASTE; SIMULATION AB The evaluation of radiation damage in materials submitted to intense irradiation is a challenging problem for the nuclear industry. Ion beams provide efficient tools to both simulate the interactions involved during the slowing-down of energetic particles and characterize the damage induced by irradiation with the channeling technique. This article presents new results and modeling regarding the disorder depth distribution and the damage build-up in nuclear materials irradiated with low- and high-energy ions which allow exploring the nuclear collision and electronic excitation regimes. A new phenomenon (SHIBIEC), leading to the recovery by electronic excitation of the damage created by ballistic collisions, is also discussed. (C) 2012 Elsevier B.V. All rights reserved. C1 [Thome, L.; Moll, S.; Debelle, A.; Garrido, F.] Univ Paris 11, Ctr Spectrometrie Nucl & Spectrometrie Masse, CNRS, IN2P3, F-91405 Orsay, France. [Moll, S.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Sattonnay, G.] Univ Paris 11, LEMHE, ICMMO, UMR 8182, F-91405 Orsay, France. [Jagielski, J.] Andrzej Soltan Inst Nucl Studies, PL-05400 Otwock, Poland. [Jagielski, J.] Inst Elect Mat Technol, PL-01919 Warsaw, Poland. RP Thome, L (reprint author), Univ Paris 11, Ctr Spectrometrie Nucl & Spectrometrie Masse, CNRS, IN2P3, Bat 108, F-91405 Orsay, France. EM thome@csnsm.in2p3.fr NR 43 TC 8 Z9 8 U1 7 U2 28 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-583X J9 NUCL INSTRUM METH B JI Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms PD NOV 1 PY 2012 VL 290 BP 6 EP 12 DI 10.1016/j.nimb.2012.08.018 PG 7 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA 042JC UT WOS:000311466500002 ER PT J AU Grinstein, FF Gowardhan, AA Ristorcelli, JR Wachtor, AJ AF Grinstein, F. F. Gowardhan, A. A. Ristorcelli, J. R. Wachtor, A. J. TI On coarse-grained simulations of turbulent material mixing SO PHYSICA SCRIPTA LA English DT Article ID LARGE-EDDY SIMULATION; RICHTMYER-MESHKOV INSTABILITY; WALL-BOUNDED FLOWS; INITIAL CONDITIONS; TAYLOR INSTABILITY; CONSERVATION-LAWS; RAYLEIGH-TAYLOR; CHANNEL FLOW; SCHEMES; RESHOCK AB Under-resolved computer simulations are typically unavoidable in many practical turbulent flow applications exhibiting extreme geometrical complexity and broad ranges of length and time scales. In such applications, coarse-grained simulation (CGS) becomes the effective simulation strategy, mostly by necessity rather than by choice. In CGS strategies, resolved/unresolved scale separation is assumed possible, large energy-containing structures are mostly resolved, smaller structures are spatially filtered out and unresolved subgrid effects are modeled; this includes classical large-eddy simulation (LES) strategies with the explicit use of closure subgrid scale models and implicit LES, relying on subgrid modeling implicitly provided by physics-capturing numerical algorithms. Predictability issues in CGS of under-resolved mixing of material scalars driven by under-resolved velocity fields and initial conditions are addressed in this paper, and shock-driven turbulent mixing is a particular focus. C1 [Grinstein, F. F.; Gowardhan, A. A.; Ristorcelli, J. R.; Wachtor, A. J.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Grinstein, FF (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM fgrinstein@lanl.gov OI Wachtor, Adam/0000-0003-0609-9171 FU US Department of Energy NNSA [DE-AC52-06NA25396]; LANL Laboratory Directed Research and Development Program on 'Turbulence by Design' through directed research project [20090058DR]; LDRD program on 'LES Modeling for Predictive Simulations of Material Mixing' through exploratory research project [20100441ER] FX We thank C Fureby, B Rider, M Andrews and K Prestridge for sharing results of their work and for very helpful and stimulating discussions. LANL is operated by the Los Alamos National Security, LLC for the US Department of Energy NNSA under contract no. DE-AC52-06NA25396. This work was made possible by funding from the LANL Laboratory Directed Research and Development Program on 'Turbulence by Design' through directed research project no. 20090058DR and from the LDRD program on 'LES Modeling for Predictive Simulations of Material Mixing' through exploratory research project no. 20100441ER. NR 87 TC 1 Z9 1 U1 0 U2 10 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0031-8949 J9 PHYS SCRIPTA JI Phys. Scr. PD NOV PY 2012 VL 86 IS 5 AR 058203 DI 10.1088/0031-8949/86/05/058203 PG 28 WC Physics, Multidisciplinary SC Physics GA 034YY UT WOS:000310910000023 ER PT J AU Smalyuk, VA AF Smalyuk, V. A. TI Experimental techniques for measuring Rayleigh-Taylor instability in inertial confinement fusion SO PHYSICA SCRIPTA LA English DT Article ID LASER-PRODUCED PLASMAS; PLANAR TARGETS; GROWTH-RATE; VALIDATION; EVOLUTION; TRANSPORT; FRONTS; SYSTEM; LIGHT; MODEL AB Rayleigh-Taylor (RT) instability is one of the major concerns in inertial confinement fusion (ICF) because it amplifies target modulations in both acceleration and deceleration phases of implosion, which leads to shell disruption and performance degradation of imploding targets. This article reviews experimental results of the RT growth experiments performed on OMEGA laser system, where targets were driven directly with laser light. RT instability was studied in the linear and nonlinear regimes. The experiments were performed in acceleration phase, using planar and spherical targets, and in deceleration phase of spherical implosions, using spherical shells. Initial target modulations consisted of two-dimensional (2D) pre-imposed modulations, and 2D and three-dimensional (3D) modulations imprinted on targets by the nonuniformities in laser drive. In planar geometry, the nonlinear regime was studied using 3D modulations with broadband spectra near nonlinear saturation levels. In acceleration-phase, the measured modulation Fourier spectra and nonlinear growth velocities are in good agreement with those predicted by Haan's model (Haan 1989 Phys. Rev. A 39 5812). In a real-space analysis, the bubble merger was quantified by a self-similar evolution of bubble size distributions (Oron et al 2001 Phys. Plasmas 8 2883). The 3D, inner-surface modulations were measured to grow throughout the deceleration phase of spherical implosions. RT growth rates are very sensitive to the drive conditions, therefore they can be used to test and validate drive physics in hydrodynamic codes used to design ICF implosions. Measured growth rates of pre-imposed 2D target modulations below nonlinear saturation levels were used to validate nonlocal thermal electron transport model in laser-driven experiments. C1 Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RP Smalyuk, VA (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. EM smalyuk2@llnl.gov FU US Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 39 TC 5 Z9 5 U1 1 U2 19 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0031-8949 J9 PHYS SCRIPTA JI Phys. Scr. PD NOV PY 2012 VL 86 IS 5 AR 058204 DI 10.1088/0031-8949/86/05/058204 PG 8 WC Physics, Multidisciplinary SC Physics GA 034YY UT WOS:000310910000024 ER PT J AU Chang, SJ Van der Lee, S Flanagan, MP AF Chang, Sung-Joon Van der Lee, Suzan Flanagan, Megan P. TI A new P-velocity model for the Tethyan margin from a scaled S-velocity model and the inversion of P- and PKP-delay times SO PHYSICS OF THE EARTH AND PLANETARY INTERIORS LA English DT Article DE P-velocity model; 3D reference model; Tethyan margin; Seismic tomography; Empirical scaling ID SPARSE LINEAR-EQUATIONS; LEAST-SQUARES; TOMOGRAPHY REVEALS; MANTLE; BENEATH; LOCATION; HOTSPOT; REGION; ZONE; LSQR AB We estimate a 3D P-velocity model for the Tethyan margin by inverting P- and PKP-delay times. The inversion is relative to a 3D reference model, which is a scaled S-velocity model for the same region. This S-velocity model was derived by jointly inverting regional S and Rayleigh waveform fits, teleseismic arrival times, Rayleigh-wave group velocities, and independent Moho constraints. Thus, our 3D reference model includes structures resolved over a larger depth range as well as more information on aseismic regions with few stations than is typically obtained from traditional teleseismic delay time inversions. We then inverted P- and PKP-delay times to obtain perturbations relative to the scaled 3D reference model. Comparing our P-velocity model (EAPV11) with P-velocity models derived from P data only, we find a model with more uniform and better depth resolution, including velocity anomalies for aseismic regions with few stations such as North Africa, southeastern Arabia, and the East European platform. Using EAPV11 to predict arrival times for relatively accurately located events that were not used in the inversion shows that our model produces significant variance reductions for these data as well. Therefore, our approach to build P-velocity models based on 3D reference S-velocity models may provide a practical way to better estimate P-velocity anomalies in the uppermost mantle and beneath aseismic regions with few stations. (c) 2012 Elsevier B.V. All rights reserved. C1 [Chang, Sung-Joon; Van der Lee, Suzan] Northwestern Univ, Dept Earth & Planetary Sci, Evanston, IL 60208 USA. [Flanagan, Megan P.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RP Chang, SJ (reprint author), Univ E Anglia, Sch Environm Sci, Norwich NR4 7TJ, Norfolk, England. EM sungjoon.chang@gmail.com RI van der Lee, Suzan/K-1144-2013; Chang, Sung-Joon/A-2114-2009 OI van der Lee, Suzan/0000-0003-1884-1185; FU Korea Research Foundation Grant [KRF-2006-214-000092]; Korean Government (MOEHRD); U.S. DOE [DE-FC52-04NA25541] FX We thank Margaret Benoit, Andy Nyblade, Yongcheol Park, and Christian Schmid for sharing their relative P arrival time data sets. We are also grateful to Bob Engdahl for access to his EHB database. Raiden Hasegawa, Ryan Lange, and Xiaoting Lou helped us to get relative arrival time data at central Asia and Turkey. We thank Stewart Fishwick and an anonymous reviewer for providing valuable suggestions that improved this manuscript. All figures were created using Generic Mapping Tools (GMT; Wessel and Smith, 1998). This work was supported by the Korea Research Foundation Grant KRF-2006-214-000092 funded by the Korean Government (MOEHRD) and the U.S. DOE under contract DE-FC52-04NA25541. NR 25 TC 1 Z9 1 U1 0 U2 3 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0031-9201 J9 PHYS EARTH PLANET IN JI Phys. Earth Planet. Inter. PD NOV PY 2012 VL 210 BP 1 EP 7 DI 10.1016/j.pepi.2012.08.005 PG 7 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA 044XM UT WOS:000311658500001 ER PT J AU Ahmed, SA Awosika, J Baldwin, C Bishop-Lilly, KA Biswas, B Broomall, S Chain, PSG Chertkov, O Chokoshvili, O Coyne, S Davenport, K Detter, JC Dorman, W Erkkila, TH Folster, JP Frey, KG George, M Gleasner, C Henry, M Hill, KK Hubbard, K Insalaco, J Johnson, S Kitzmiller, A Krepps, M Lo, CC Luu, T McNew, LA Minogue, T Munk, CA Osborne, B Patel, M Reitenga, KG Rosenzweig, CN Shea, A Shen, XH Strockbine, N Tarr, C Teshima, H van Gieson, E Verratti, K Wolcott, M Xie, G Sozhamannan, S Gibbons, HS AF Ahmed, Sanaa A. Awosika, Joy Baldwin, Carson Bishop-Lilly, Kimberly A. Biswas, Biswajit Broomall, Stacey Chain, Patrick S. G. Chertkov, Olga Chokoshvili, Otar Coyne, Susan Davenport, Karen Detter, J. Chris Dorman, William Erkkila, Tracy H. Folster, Jason P. Frey, Kenneth G. George, Matroner Gleasner, Cheryl Henry, Matthew Hill, Karen K. Hubbard, Kyle Insalaco, Joseph Johnson, Shannon Kitzmiller, Aaron Krepps, Michael Lo, Chien-Chi Truong Luu McNew, Lauren A. Minogue, Timothy Munk, Christine A. Osborne, Brian Patel, Mohit Reitenga, Krista G. Rosenzweig, C. Nicole Shea, April Shen, Xiaohong Strockbine, Nancy Tarr, Cheryl Teshima, Hazuki van Gieson, Eric Verratti, Kathleen Wolcott, Mark Xie, Gary Sozhamannan, Shanmuga Gibbons, Henry S. CA Threat Characterization Consortium TI Genomic Comparison of Escherichia coli O104:H4 Isolates from 2009 and 2011 Reveals Plasmid, and Prophage Heterogeneity, Including Shiga Toxin Encoding Phage stx2 SO PLOS ONE LA English DT Article ID HEMOLYTIC-UREMIC SYNDROME; SALMONELLA-TYPHIMURIUM; AGGREGATIVE ADHERENCE; GADE YHIE; BACTERIOPHAGES; RESISTANCE; PATHOGENS; SEQUENCES; ALIGNMENT; OUTBREAK AB In May of 2011, an enteroaggregative Escherichia coli O104:H4 strain that had acquired a Shiga toxin 2-converting phage caused a large outbreak of bloody diarrhea in Europe which was notable for its high prevalence of hemolytic uremic syndrome cases. Several studies have described the genomic inventory and phylogenies of strains associated with the outbreak and a collection of historical E. coli O104: H4 isolates using draft genome assemblies. We present the complete, closed genome sequences of an isolate from the 2011 outbreak (2011C-3493) and two isolates from cases of bloody diarrhea that occurred in the Republic of Georgia in 2009 (2009EL-2050 and 2009EL-2071). Comparative genome analysis indicates that, while the Georgian strains are the nearest neighbors to the 2011 outbreak isolates sequenced to date, structural and nucleotide-level differences are evident in the Stx2 phage genomes, the mer/tet antibiotic resistance island, and in the prophage and plasmid profiles of the strains, including a previously undescribed plasmid with homology to the pMT virulence plasmid of Yersinia pestis. In addition, multiphenotype analysis showed that 2009EL-2071 possessed higher resistance to polymyxin and membrane-disrupting agents. Finally, we show evidence by electron microscopy of the presence of a common phage morphotype among the European and Georgian strains and a second phage morphotype among the Georgian strains. The presence of at least two stx2 phage genotypes in host genetic backgrounds that may derive from a recent common ancestor of the 2011 outbreak isolates indicates that the emergence of stx2 phage-containing E. coli O104: H4 strains probably occurred more than once, or that the current outbreak isolates may be the result of a recent transfer of a new stx2 phage element into a pre-existing stx2-positive genetic background. C1 [Broomall, Stacey; Hubbard, Kyle; Insalaco, Joseph; Krepps, Michael; McNew, Lauren A.; Rosenzweig, C. Nicole; Gibbons, Henry S.] USA, Edgewood Chem Biol Ctr, Aberdeen Proving Ground, MD USA. [Ahmed, Sanaa A.; Chain, Patrick S. G.; Chertkov, Olga; Davenport, Karen; Detter, J. Chris; Erkkila, Tracy H.; Gleasner, Cheryl; Hill, Karen K.; Johnson, Shannon; Lo, Chien-Chi; Munk, Christine A.; Reitenga, Krista G.; Shen, Xiaohong; Teshima, Hazuki; Xie, Gary] Los Alamos Natl Lab, Los Alamos, NM USA. [Awosika, Joy; Bishop-Lilly, Kimberly A.; Biswas, Biswajit; Frey, Kenneth G.; George, Matroner; Henry, Matthew; Truong Luu; Patel, Mohit; Verratti, Kathleen; Sozhamannan, Shanmuga] USN, Med Res Ctr, Frederick, MD USA. [Awosika, Joy; Bishop-Lilly, Kimberly A.; Biswas, Biswajit; Frey, Kenneth G.; George, Matroner; Henry, Matthew; Truong Luu; Patel, Mohit; Verratti, Kathleen; Sozhamannan, Shanmuga] Henry M Jackson Fdn Mil Med, Frederick, MD USA. [Baldwin, Carson; Coyne, Susan; Dorman, William; Minogue, Timothy; Shea, April; Wolcott, Mark] USA, Res Inst Infect Dis, Frederick, MD USA. [Chokoshvili, Otar] Natl Ctr Dis Control & Publ Hlth, S Caucasus Field Epidemiol & Lab Training Program, Tbilisi, Rep of Georgia. [Folster, Jason P.; Strockbine, Nancy; Tarr, Cheryl] Ctr Dis Control & Prevent, Enter Dis Lab Branch, Atlanta, GA USA. [Hubbard, Kyle; Krepps, Michael] Excet Inc, Springfield, VA USA. [Insalaco, Joseph] Sci Applicat Int Corp, Abingdon, MD USA. [Kitzmiller, Aaron; Osborne, Brian] BioTeam Inc, Middleton, MA USA. [Shea, April] Team Keaki Tech, Frederick, MD USA. [van Gieson, Eric] Def Threat Reduct Agcy, Alexandria, VA USA. RP Gibbons, HS (reprint author), USA, Edgewood Chem Biol Ctr, Aberdeen Proving Ground, MD USA. EM henry.s.gibbons.civ@mail.mil RI chain, patrick/B-9777-2013; OI Johnson, Shannon/0000-0002-3972-9208; Chain, Patrick/0000-0003-3949-3634; xie, gary/0000-0002-9176-924X FU Defense Threat Reduction Agency [CB2847, IB06RSQ002] FX The work presented here was supported by the Defense Threat Reduction Agency (www.dtra.mil) Transformational Medical Technologies program under project numbers CB2847 to HSG and CNR; IB06RSQ002 to SS; and to JCD. The funding agency participated in the formation of the consortium but did not impact the collection of data, analysis, decision to publish, or preparation of the manuscript. NR 90 TC 38 Z9 40 U1 1 U2 36 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD NOV 1 PY 2012 VL 7 IS 11 AR e48228 DI 10.1371/journal.pone.0048228 PG 22 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA 030WR UT WOS:000310601300006 PM 23133618 ER PT J AU Wang, L Swensen, JS AF Wang, Liang Swensen, James S. TI Dual-transduction-mode sensing approach for chemical detection SO SENSORS AND ACTUATORS B-CHEMICAL LA English DT Article DE Dual-modal sensor; Chemical; Light-emitting OFET ID ELECTRONIC-NOSE TECHNOLOGIES; VOLATILE ORGANIC-COMPOUNDS; COLORIMETRIC SENSOR ARRAY; FIELD-EFFECT TRANSISTORS; EXHALED BREATH; LUNG-CANCER; CONJUGATED POLYMERS; CARBON NANOTUBES; CARRIER MOBILITY; DISCRIMINATION AB Smart devices such as electronic nose have been developed for application in many fields like national security, defense, environmental regulation, health care, pipeline monitoring and food analysis. Despite a large array of individual sensors, the resolving power of these devices can still be improved to identify a target at a very low concentration out of a mixture of odors, if different types of transductions are employed in concert as a set of sensing responses to distinguish one odor from another. Here, we propose a new sensor architecture enabling different types of transduction signals in parallel on the same individual sensor. We demonstrate this architecture using a light emitting organic field-effect transistor (LEOFET) operated at a dual-transduction mode, as a proof-of-concept. Sensing response has been observed on both electrical and optical output signals from a green LEOFET upon exposure to an explosive taggant, with optical signal exhibiting much higher sensitivity. This new sensor architecture opens a field of devices of synergic capabilities to distinguish chemical and biological targets. (c) 2012 Elsevier B.V. All rights reserved. C1 [Wang, Liang; Swensen, James S.] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99354 USA. RP Swensen, JS (reprint author), Pacific NW Natl Lab, Energy & Environm Directorate, 902 Battelle Blvd,POB 999,MSIN K3-59, Richland, WA 99354 USA. EM james.swensen@pnnl.gov FU Laboratory Directed Research and Development Program at the Pacific Northwest National Laboratory [PN09049/2217] FX This work was supported by the Laboratory Directed Research and Development Program at the Pacific Northwest National Laboratory (Project Identifier PN09049/2217). L.W. and J.S.S. contributed equally to this work. Fig. S2 was generated as part of the dissertation research of J.S.S. We thank Professor Alan J. Heeger for his help and advice in generating the data shown in Fig. S2. NR 64 TC 5 Z9 5 U1 5 U2 43 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0925-4005 J9 SENSOR ACTUAT B-CHEM JI Sens. Actuator B-Chem. PD NOV PY 2012 VL 174 BP 366 EP 372 DI 10.1016/j.snb.2012.08.036 PG 7 WC Chemistry, Analytical; Electrochemistry; Instruments & Instrumentation SC Chemistry; Electrochemistry; Instruments & Instrumentation GA 040NG UT WOS:000311329000053 ER PT J AU Daughton, W Roytershteyn, V AF Daughton, William Roytershteyn, Vadim TI Emerging Parameter Space Map of Magnetic Reconnection in Collisional and Kinetic Regimes SO SPACE SCIENCE REVIEWS LA English DT Review DE Magnetic; Reconnection; Plasmoids ID IMPULSIVE RECONNECTION; SOLAR-FLARE; PLASMA; SIMULATIONS; CHALLENGE; JETS; CODE AB In large-scale systems of interest to solar physics, there is growing evidence that magnetic reconnection involves the formation of extended current sheets which are unstable to plasmoids (secondary magnetic islands). Recent results suggest that plasmoids may play a critical role in the evolution of reconnection, and have raised fundamental questions regarding the applicability of resistive MHD to various regimes. In collisional plasmas, where the thickness of all resistive layers remain larger than the ion gyroradius, simulations results indicate that plasmoids permit reconnection to proceed much faster than the slow Sweet-Parker scaling. However, it appears these rates are still a factor of similar to 10x slower than observed in kinetic regimes, where the diffusion region current sheet falls below the ion gyroradius and additional physics beyond MHD becomes crucially important. Over a broad range of interesting parameters, the formation of plasmoids may naturally induce a transition into these kinetic regimes. New insights into this scenario have emerged in recent years based on a combination of linear theory, fluid simulations and fully kinetic simulations which retain a Fokker-Planck collision operator to allow a rigorous treatment of Coulomb collisions as the reconnection electric field exceeds the runaway limit. Here, we present some new results from this approach for guide field reconnection. Based upon these results, a parameter space map is constructed that summarizes the present understanding of how reconnection proceeds in various regimes. C1 [Daughton, William; Roytershteyn, Vadim] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Daughton, W (reprint author), Los Alamos Natl Lab, MS F699, Los Alamos, NM 87545 USA. EM daughton@lanl.gov; roytersh@lanl.gov RI Daughton, William/L-9661-2013; OI Roytershteyn, Vadim/0000-0003-1745-7587 FU U.S. Department of Energy through the LANL/LDRD Program; Institutional Computing Program at Los Alamos FX We gratefully acknowledge support from the U.S. Department of Energy through the LANL/LDRD Program and from the Institutional Computing Program at Los Alamos. NR 62 TC 22 Z9 22 U1 0 U2 15 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0038-6308 EI 1572-9672 J9 SPACE SCI REV JI Space Sci. Rev. PD NOV PY 2012 VL 172 IS 1-4 BP 271 EP 282 DI 10.1007/s11214-011-9766-z PG 12 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 034MJ UT WOS:000310877300018 ER PT J AU Camporeale, E AF Camporeale, Enrico TI Nonmodal Linear Theory for Space Plasmas SO SPACE SCIENCE REVIEWS LA English DT Review DE Solar wind; Linear theory ID ELECTRON-TEMPERATURE ANISOTROPY; SOLAR-WIND; SHEAR FLOWS; STABILITY THEORY; MAGNETOHYDRODYNAMIC WAVES; BYPASS TRANSITION; TRANSFORMATIONS AB The nonmodal approach is a linear theory formalism that emphasizes the transient evolution of a perturbed equilibrium. It differs from the normal-mode analysis by not assuming an exponential behavior of physical perturbations. We discuss works that have applied the nonmodal formalism to the problem of solar wind heating and acceleration. We briefly review the methodology of the Kelvin formalism and of the Generalized Stability Theory, and discuss the cases of both sheared and non-sheared plasmas. The results and methodology reviewed in this paper could form the basis for a trend of research in solar wind dynamics that has not been yet systematically explored. C1 Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Camporeale, E (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM enrico@lanl.gov FU STFC [ST/H002731/1] FX I acknowledge the kind hospitality of the International Space Science Institute (Bern), and I would like to thank Gian Luca Delzanno and David Burgess for useful discussions on the topic of nonmodal linear theory. This work was partially supported by STFC grant ST/H002731/1. NR 36 TC 5 Z9 5 U1 1 U2 10 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0038-6308 J9 SPACE SCI REV JI Space Sci. Rev. PD NOV PY 2012 VL 172 IS 1-4 BP 397 EP 409 DI 10.1007/s11214-011-9764-1 PG 13 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 034MJ UT WOS:000310877300026 ER PT J AU Chia, CC Jeong, HM Lee, JR Park, G AF Chia, Chen Ciang Jeong, Hyo-Mi Lee, Jung-Ryul Park, Gyuhae TI Composite aircraft debonding visualization by laser ultrasonic scanning excitation and integrated piezoelectric sensing SO STRUCTURAL CONTROL & HEALTH MONITORING LA English DT Article DE laser ultrasonic propagation imaging; nondestructive evaluation; structural health monitoring; poor bonding defect; real debonding damages; complex composite structures ID LAMB WAVES; DAMAGE; PROPAGATION; TRANSDUCER; GENERATION; VIBROMETRY; ALUMINUM; SYSTEM; PLATES AB Two aircraft wings made of carbon fiber-reinforced plastic material were inspected using the laser-based ultrasonic propagation imaging system for the visualization of manufacturing defect and damages of debonding mode. Hypotheses of the detection mechanism of composite debonding were presented and validated through the inspection results for the bonding lines of the composite wing structures. The inspection showed that the location, shape, and size of the poor bonding defect, artificial stringer tip debonding, and real skinspar debonding can be visualized and/or measured from the imaging results. The performance of the imaging system was found better than that of a manual ultrasonic C-scan in terms of spatial resolution and damage detectability. Another finding from the inspection was the occurrence of skin buckling between two riveted locations. Most importantly, the presence of structural elements or features such as spars, stringers, ribs, lugs, inspection windows, and even embedded PZT elements did not adversely affect the inspection. Copyright (C) 2012 John Wiley & Sons, Ltd. C1 [Chia, Chen Ciang; Jeong, Hyo-Mi; Lee, Jung-Ryul] Chonbuk Natl Univ, Dept Aerosp Engn, Jeonju Si 561756, Jeollabuk Do, South Korea. [Chia, Chen Ciang; Jeong, Hyo-Mi; Lee, Jung-Ryul] Chonbuk Natl Univ, LANL CBNU Engn Inst Korea, Jeonju Si 561756, Jeollabuk Do, South Korea. [Park, Gyuhae] Los Alamos Natl Lab, Engn Inst, Los Alamos, NM 87545 USA. RP Lee, JR (reprint author), Chonbuk Natl Univ, Dept Aerosp Engn, 567 Baekje Daero, Jeonju Si 561756, Jeollabuk Do, South Korea. EM leejrr@jbnu.ac.kr RI Lee, Jung-Ryul/B-3266-2015; OI Chia, Chen Ciang/0000-0003-0384-7648 FU ADD (Agency for Defense Development) in Korea [UC080019JD]; Leading Foreign Research Institute Recruitment Program through the National Research Foundation of Korea; Basic Science Research Program through the National Research Foundation of Korea [2011-0010489]; Ministry of Education, Science and Technology; Ministry of Land, Transport and Maritime Affairs as Haneul Project FX We performed this study under the applied research project (UC080019JD), which is supported by ADD (Agency for Defense Development) in Korea. This research was also supported by Leading Foreign Research Institute Recruitment Program (2011) and Basic Science Research Program (2011-0010489) through the National Research Foundation of Korea, funded by the Ministry of Education, Science and Technology and by the Ministry of Land, Transport and Maritime Affairs as Haneul Project. NR 44 TC 5 Z9 5 U1 0 U2 31 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1545-2255 EI 1545-2263 J9 STRUCT CONTROL HLTH JI Struct. Control. Health Monit. PD NOV PY 2012 VL 19 IS 7 SI SI BP 605 EP 620 DI 10.1002/stc.1504 PG 16 WC Construction & Building Technology; Engineering, Civil; Instruments & Instrumentation SC Construction & Building Technology; Engineering; Instruments & Instrumentation GA 041JC UT WOS:000311396800006 ER PT J AU Shin, HJ Yun, CY Park, G Farinholt, KM Lee, JR Park, CY Jun, SM Farrar, CR AF Shin, Hye-Jin Yun, Chang-Yong Park, Gyuhae Farinholt, Kevin M. Lee, Jung-Ryul Park, Chan-Yik Jun, Seung-Moon Farrar, Charles R. TI Assessing joint integrity of a lug assembly using piezoelectric active sensors SO STRUCTURAL CONTROL & HEALTH MONITORING LA English DT Article DE structural health monitoring; piezoelectric active sensor; frequency response function; time-series models; bolted joint ID DAMAGE DETECTION; HEALTH; WAVES AB This paper is a report of an investigation into tracking and monitoring the integrity of bolted joints using piezoelectric active sensors. The target application of this study is a fitting lug assembly of unmanned aerial vehicles (UAVs), where a composite wing is mounted to a UAV fuselage. The structural health monitoring methods deployed in this study are time-series analysis and high-frequency response functions measured by piezoelectric active sensors. Different types of simulated damage are introduced into the structure, and the capability of each technique is examined. Practical implementation issues, including temperature changes, are also considered in this study. The results collected from the tests show that piezoelectric active sensors and associated signal processing tools can be efficiently used for identifying joint failure modes of a lug assembly. Copyright (C) 2012 John Wiley & Sons, Ltd. C1 [Park, Gyuhae; Farinholt, Kevin M.; Farrar, Charles R.] Chonnam Natl Univ, Sch Mech Syst Engn, Kwangju 500757, South Korea. [Shin, Hye-Jin; Yun, Chang-Yong; Lee, Jung-Ryul] Chonbuk Natl Univ, Dept Aerosp Engn, Jeonju 561756, Jeollabuk Do, South Korea. [Shin, Hye-Jin; Yun, Chang-Yong; Lee, Jung-Ryul] Chonbuk Natl Univ, LANL CBNU Engn Inst Korea, Jeonju 561756, Jeollabuk Do, South Korea. [Park, Gyuhae; Farinholt, Kevin M.; Farrar, Charles R.] Los Alamos Natl Lab, Engn Inst, Los Alamos, NM 87545 USA. [Park, Chan-Yik; Jun, Seung-Moon] Agcy Def Dev, R&D Inst 7, Airframe Technol Directorate, Taejon 305600, South Korea. RP Park, G (reprint author), Chonnam Natl Univ, Sch Mech Syst Engn, Kwangju 500757, South Korea. EM gpark@jnu.ac.kr RI Lee, Jung-Ryul/B-3266-2015; OI Farrar, Charles/0000-0001-6533-6996 FU Laboratory Directed Research and Development program at Los Alamos National Laboratory; Leading Foreign Research Institute Recruitment Program through the National Research Foundation of Korea; Ministry of Education, Science and Technology [2011-0030065] FX This research was funded through the Laboratory Directed Research and Development program at Los Alamos National Laboratory. This research was also partially supported by the Leading Foreign Research Institute Recruitment Program through the National Research Foundation of Korea funded by the Ministry of Education, Science and Technology (2011-0030065). NR 26 TC 5 Z9 5 U1 0 U2 8 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1545-2255 EI 1545-2263 J9 STRUCT CONTROL HLTH JI Struct. Control. Health Monit. PD NOV PY 2012 VL 19 IS 7 SI SI BP 621 EP 631 DI 10.1002/stc.1507 PG 11 WC Construction & Building Technology; Engineering, Civil; Instruments & Instrumentation SC Construction & Building Technology; Engineering; Instruments & Instrumentation GA 041JC UT WOS:000311396800007 ER PT J AU Patlolla, A Carino, EV Ehrlich, SN Stavitski, E Frenkel, AI AF Patlolla, A. Carino, E. V. Ehrlich, S. N. Stavitski, E. Frenkel, A. I. TI Application of Operando XAS, XRD, and Raman Spectroscopy for Phase Speciation in Water Gas Shift Reaction Catalysts SO ACS CATALYSIS LA English DT Article DE catalysis; in situ; operando; combined techniques; XANES; EXAFS; XRD; Raman spectroscopy ID X-RAY-ABSORPTION; IN-SITU CHARACTERIZATION; ACTIVE-SITES; TEMPERATURE; CHROMIUM; COPPER; CRYSTALLINE; MAGNETITE; CELL; CU AB The structural and compositional changes of the partially reduced iron oxide Fe2O3 and 3% chromium oxide-modified iron oxide (3% Cr2O3/Fe2O3) catalysts before, during, and after the water gas shift (WGS) reaction are reported. The measurements were performed by collecting X-ray absorption fine structure, X-ray diffraction, and Raman. spectroscopy data on the catalysts and the mass spectrometry data of reactants and products, all done in a single experiment. These materials demonstrated marked structural disorder and compositional heterogeneity that are peaked in their catalytically active states. The main findings revealed in the result of combining multiple techniques include the role of Cr in stabilizing the low-temperature gamma-Fe2O3 phase, the nature of the disordered phase in the active state of the catalysts, and the possible deactivation mechanism. C1 [Ehrlich, S. N.; Stavitski, E.] Brookhaven Natl Lab, Natl Synchrotron Light Source, Upton, NY 11973 USA. [Patlolla, A.; Frenkel, A. I.] Yeshiva Univ, Dept Phys, New York, NY 10016 USA. [Carino, E. V.] Univ Delaware, Dept Chem Engn, Newark, DE 19716 USA. RP Stavitski, E (reprint author), Brookhaven Natl Lab, Natl Synchrotron Light Source, Upton, NY 11973 USA. EM istavitski@bnl.gov; anatoly.frenkel@yu.edu RI Frenkel, Anatoly/D-3311-2011; Stavitski, Eli/C-4863-2009 OI Frenkel, Anatoly/0000-0002-5451-1207; FU U.S. Department of Energy (DOE) [DE-FG02-03ER15476, DE-FG02-05ER15688, DE-AC02-98CH10866]; Synchrotron Catalysis Consortium (U.S. DOE) [DE-FG02-05ER15688] FX The authors are grateful to Prof. I. Wachs and C. Keturakis for sample preparation and for useful discussions and to Dr. Q Wang for beamline support. A.I.F. and A.P. acknowledge the support of this work by the U.S. Department of Energy (DOE), Grant No. DE-FG02-03ER15476. E.C. is supported by the Synchrotron Catalysis Consortium (U.S. DOE Grant No. DE-FG02-05ER15688). Beamline X18A is supported in part by the U.S. DOE Grant No. DE-FG02-05ER15688. NSLS is supported by the U.S. DOE Grant No. DE-AC02-98CH10866. NR 69 TC 17 Z9 17 U1 4 U2 77 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2155-5435 J9 ACS CATAL JI ACS Catal. PD NOV PY 2012 VL 2 IS 11 BP 2216 EP 2223 DI 10.1021/cs300414c PG 8 WC Chemistry, Physical SC Chemistry GA 032MT UT WOS:000310723900001 ER PT J AU Wu, ZL Li, MJ Mullins, DR Overbury, SH AF Wu, Zili Li, Meijun Mullins, David R. Overbury, Steven H. TI Probing the Surface Sites of CeO2 Nanocrystals with Well-Defined Surface Planes via Methanol Adsorption and Desorption SO ACS CATALYSIS LA English DT Article DE ceria nanoshapes; rods; cubes; octahedra; surface sites; methanol adsorption and desorption; in situ spectroscopy ID DENSITY-FUNCTIONAL THEORY; TEMPERATURE CO OXIDATION; IR MOLECULAR PROBE; GAS SHIFT REACTION; CERIUM OXIDE; ROOM-TEMPERATURE; OXYGEN STORAGE; INFRARED-SPECTROSCOPY; AU/SIO2 CATALYST; NANORODS AB Methanol has been considered as a "smart" molecule in studying the surface sites of metal oxide catalysts. In this work, methanol was utilized to probe the nature of surface sites of ceria nanocrystals with defined surface planes (nanoshapes), including rods (containing {110}), cubes ({100}), and octahedra ({111}). The adsorption and desorption of methanol were followed by in situ IR and Raman spectroscopy as well as mass spectrometry. Upon methanol adsorption at room temperature, on-top, bridging and three-coordinate methoxy species are formed on the surface of rods and cubes, whereas only on-top methoxy is present on the octahedra surface. The distribution of the methoxy species is believed to be determined not only by the coordination status of surface Ce cations but also by the number of defect sites on the three nanoshapes. During the desorption process, the methoxy species are gradually dehydrogenated into H-2 and CO via formate species as intermediates on the three ceria surfaces A second intermediate, formyl species is also evident on the rods surface. The methoxy species are more reactive and less stable on the rods' surface, which results in desorption of H-2 and CO at lower temperature (<583 K) than on cubes and octahedra. A higher than stoichiometric H/CO ratio is observed in the methanol-TPD products, attributed to the retention of some amount of formate and carbonate species on the ceria nanoshapes, as revealed by in situ IR. A small amount of methanol and formaldehyde desorbs at low temperature (<423 K) on the three surfaces as a result of the disproportionation reaction of the methoxy species. The UV Raman and IR results indicate that the ceria nanoshapes are slightly reduced at room temperature upon methanol adsorption and become more reduced at higher temperatures during methanol desorption. The degree of reduction is found to be dependent on the surface structure of the ceria nanoshapes. C1 [Wu, Zili; Li, Meijun; Mullins, David R.; Overbury, Steven H.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Wu, Zili; Overbury, Steven H.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Wu, ZL (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. EM wuz1@ornl.gov; overburysh@ornl.gov RI Wu, Zili/F-5905-2012; Overbury, Steven/C-5108-2016 OI Wu, Zili/0000-0002-4468-3240; Overbury, Steven/0000-0002-5137-3961 FU Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy; Oak Ridge National Laboratory by the Scientific User Facility Division, Office of Basic Energy Science, U.S. Department of Energy; ORNL; Oak Ridge Associated Universities FX This Research is sponsored by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy. Part of the work, including the Raman study, was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facility Division, Office of Basic Energy Science, U.S. Department of Energy. The research was supported in part by the appointment for M.J.L. to the ORNL Postdoctoral Research Associates Program, administered jointly by ORNL and the Oak Ridge Associated Universities. NR 51 TC 53 Z9 53 U1 18 U2 189 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2155-5435 J9 ACS CATAL JI ACS Catal. PD NOV PY 2012 VL 2 IS 11 BP 2224 EP 2234 DI 10.1021/cs300467p PG 11 WC Chemistry, Physical SC Chemistry GA 032MT UT WOS:000310723900002 ER PT J AU Lee, AF Naughton, JN Liu, Z Wilson, K AF Lee, Adam F. Naughton, James N. Liu, Zhi Wilson, Karen TI High-Pressure XPS of Crotyl Alcohol Selective Oxidation over Metallic and Oxidized Pd(111) SO ACS CATALYSIS LA English DT Article DE selective oxidation; palladium; high-pressure XPS; alcohol; in situ ID RAY PHOTOELECTRON-SPECTROSCOPY; SITU X-RAY; IN-SITU; AEROBIC OXIDATION; AMBIENT-PRESSURE; PD; PALLADIUM; CATALYSTS; SURFACES; PT(111) AB Here, we report on the first application of high-pressure XPS (HP-XPS) to the surface catalyzed selective oxidation of a hydrocarbon over palladium, wherein the reactivity of metal and oxide surfaces in directing the oxidative dehydrogenation of crotyl alcohol (CrOH) to crotonaldehyde (CrHCO) is evaluated. Crotonaldehyde formation is disfavored over Pd(111) under all reaction conditions, with only crotyl alcohol decomposition observed. In contrast, 2D Pd5O4 and 3D PdO overlayers are able to selectively oxidize crotyl alcohol (1 mTorr) to crotonaldehrde in the presence of co-fed oxygen (140 mTorr) at temperatures as low as 40 degrees C. However, 2D Pd5O4 ultrathin films are unstable toward reduction by the alcohol at ambient temperature, whereas the 3D PdO oxide is able to sustain catalytic crotonaldehyde production even up to 150 degrees C. Co fed oxygen is essential to stabilize palladium surface oxides toward in situ reduction by crotyl alcohol, with stability increasing with oxide film dimensionality. C1 [Lee, Adam F.; Wilson, Karen] Cardiff Univ, Sch Chem, Cardiff Catalysis Inst, Cardiff CF10 3AT, S Glam, Wales. [Naughton, James N.] Univ York, Dept Chem, York YO10 5DD, N Yorkshire, England. [Liu, Zhi] Lawrence Berkeley Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Lee, AF (reprint author), Cardiff Univ, Sch Chem, Cardiff Catalysis Inst, Cardiff CF10 3AT, S Glam, Wales. EM Leeaf@cardiff.ac.uk; Wilsonk5@cardiff.ac.uk RI Karen, Wilson/A-1061-2009; Lee, Adam/D-1162-2009; Liu, Zhi/B-3642-2009 OI Karen, Wilson/0000-0003-4873-708X; Lee, Adam/0000-0002-2153-1391; Liu, Zhi/0000-0002-8973-6561 FU EPSRC [EP/F063423/2, EP/G007594/2]; Royal Society; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX We thank the EPSRC for funding (EP/F063423/2), the award of a studentship to J.N.N., and a Leadership Fellowship (EP/G007594/2) to A.F.L. K.W. acknowledges The Royal Society for the award of an Industry Fellowship. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 44 TC 15 Z9 15 U1 1 U2 55 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2155-5435 J9 ACS CATAL JI ACS Catal. PD NOV PY 2012 VL 2 IS 11 BP 2235 EP 2241 DI 10.1021/cs300450y PG 7 WC Chemistry, Physical SC Chemistry GA 032MT UT WOS:000310723900003 ER PT J AU Alayoglu, S Krier, JM Michalak, WD Zhu, ZW Gross, E Somorjai, GA AF Alayoglu, Selim Krier, James M. Michalak, William D. Zhu, Zhongwei Gross, Elad Somorjai, Gabor A. TI In Situ Surface and Reaction Probe Studies with Model Nanoparticle Catalysts SO ACS CATALYSIS LA English DT Article DE colloidal nanoparticle catalysts; in situ surface probes; surface sum frequency generation vibrational spectroscopy; ambient pressure x-ray photoelectron spectroscopy; near edge x-ray absorption fine structure; oxidation states; elemental composition; catalytic reactivity measurements ID SUM-FREQUENCY GENERATION; RAY-ABSORPTION SPECTROSCOPY; VIBRATIONAL SPECTROSCOPY; ELECTRON-MICROSCOPY; HIGH-PRESSURES; CO OXIDATION; AMBIENT-PRESSURE; CYCLOHEXENE DEHYDROGENATION; BIMETALLIC NANOPARTICLES; ETHYLENE HYDROGENATION AB This review paper discusses the in situ surface characterization and catalytic measurements of colloidally synthesized model metal nanoparticle (NP) catalysts studied in the Somorjai lab. Sum Frequency Generation (SFG) vibrational spectroscopy technique revealed the vibrational signatures of binding geometry and surface orientation of adsorbate molecules by probing the immediate surface structure during the catalytic reactions. Metal surfaces were studied by Synchrotron-based spectroscopic techniques at the Advanced Light Source in the Lawrence Berkeley National Laboratory. Ambient Pressure X-ray Photoelectron Spectroscopy (APXPS) was employed to measure chemical and elemental structure of bimetallic NP catalysts under the catalytically relevant pressures in the Torr range. Surface chemical structure (i.e., oxidation states) of metals was obtained by X-ray Absorption Fine Structure Spectroscopy by constructing a gas flow cell that operates under atmospheric pressures as the reaction occurs. Environmental Transmission Electron Microscopy (E-TEM) supplemented the bimetallic structure that was obtained by X-ray spectroscopies. The morphology and chemistry induced by gas reactants on the stepped single crystal surfaces as determined by high-pressure in situ Scanning Tunneling Microscopy (HPSTM) and APXPS were also described. C1 [Alayoglu, Selim; Krier, James M.; Michalak, William D.; Zhu, Zhongwei; Gross, Elad; Somorjai, Gabor A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Alayoglu, Selim; Krier, James M.; Michalak, William D.; Gross, Elad; Somorjai, Gabor A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Zhu, Zhongwei; Somorjai, Gabor A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Somorjai, GA (reprint author), Univ Calif Berkeley, Dept Chem, Hildebrand Hall, Berkeley, CA 94720 USA. EM somorjai@berkeley.edu RI Foundry, Molecular/G-9968-2014 FU Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering of the U.S. Department of Energy [DE-AC02-05cH11231] FX The work shown in this review article was supported by the Director, Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering of the U.S. Department of Energy under Contract No. DE-AC02-05cH11231. NR 70 TC 19 Z9 19 U1 4 U2 108 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2155-5435 J9 ACS CATAL JI ACS Catal. PD NOV PY 2012 VL 2 IS 11 BP 2250 EP 2258 DI 10.1021/cs3004903 PG 9 WC Chemistry, Physical SC Chemistry GA 032MT UT WOS:000310723900006 ER PT J AU Frenkel, AI Rodriguez, JA Chen, JGG AF Frenkel, Anatoly I. Rodriguez, Jose A. Chen, Jingguang G. TI Synchrotron Techniques for In Situ Catalytic Studies: Capabilities, Challenges, and Opportunities SO ACS CATALYSIS LA English DT Article DE synchrotron; in situ; operando; catalysis; EXAFS; XRD ID X-RAY-ABSORPTION; GAS SHIFT CATALYSTS; REFLECTANCE INFRARED-SPECTROSCOPY; SUPPORTED PD NANOPARTICLES; ENERGY-DISPERSIVE EXAFS; ACTIVE-SITE; HETEROGENEOUS CATALYSIS; OPERANDO SPECTROSCOPY; HYDROGEN-PRODUCTION; REACTION-MECHANISM AB Most industrial catalysts are complex materials that usually operate at elevated pressures and temperatures Pressure, materials, instrument; and complexity gaps are obstacles toward understanding how catalysts work and how to rationally design new catalysts. In this article, we examine existing and emerging approaches to bridge some of these gaps and gain new insights into the catalyst active phase and catalytic mechanism using synchrotron-based spectroscopy, scattering, and imaging methods. The utilization of in situ, time-resolved synchrotron techniques offers unique opportunities to study working (operando) catalysts. Using several representative examples from recent literature we illustrate the synergy from using combinations of techniques to identify new details about catalytic properties that are unavailable when these methods are used separately. Following this approach it is possible to identify new catalyst phases and reaction intermediates. C1 [Frenkel, Anatoly I.] Yeshiva Univ, Dept Phys, New York, NY 10016 USA. [Rodriguez, Jose A.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Chen, Jingguang G.] Univ Delaware, Dept Chem Engn, Newark, DE 19716 USA. [Chen, Jingguang G.] Columbia Univ, Dept Chem Engn, New York, NY 10027 USA. RP Frenkel, AI (reprint author), Yeshiva Univ, Dept Phys, New York, NY 10016 USA. EM anatoly.frenkel@yu.edu; rodrigez@bnl.gov; jgchen@udel.edu RI Frenkel, Anatoly/D-3311-2011 OI Frenkel, Anatoly/0000-0002-5451-1207 FU U.S. Department of Energy [DE-FG02-05ER15688] FX This work was supported by the U.S. Department of Energy Grant DE-FG02-05ER15688. NR 102 TC 32 Z9 32 U1 16 U2 130 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2155-5435 J9 ACS CATAL JI ACS Catal. PD NOV PY 2012 VL 2 IS 11 BP 2269 EP 2280 DI 10.1021/cs3004006 PG 12 WC Chemistry, Physical SC Chemistry GA 032MT UT WOS:000310723900008 ER PT J AU Tupy, SA Karim, AM Bagia, C Deng, WH Huang, YL Vlachos, DG Chen, JGG AF Tupy, Sarah A. Karim, Ayman M. Bagia, Christina Deng, Weihua Huang, Yulin Vlachos, Dionisios G. Chen, Jingguang G. TI Correlating Ethylene Glycol Reforming Activity with In Situ EXAFS Detection of Ni Segregation in Supported NiPt Bimetallic Catalysts SO ACS CATALYSIS LA English DT Article DE In situ EXAFS; NiPt; ethylene glycol; supported catalysts; aqueous phase reforming; reverse Monte Carlo ID X-RAY-ABSORPTION; PLATINUM CATALYSTS; RENEWABLE HYDROGEN; REACTION-KINETICS; H-2 PRODUCTION; SURFACES; GLYCEROL; REACTIVITY; NI/PT(111); STABILITY AB The structural changes in supported NiPt/C and NiPt/gamma-Al2O3 catalysts were investigated using in situ extended X-ray absorption fine structure (EXAFS) under aqueous phase reforming (APR) of ethylene glycol conditions. Reverse Monte Carlo is introduced to analyze the EXAFS data. Parallel reactor studies of APR of ethylene glycol showed that NiPt catalysts were initially more active than monometallic Pt catalysts. The enhanced activity was correlated to changes in the catalyst structure. Under APR conditions, Ni segregated to the surface of the catalysts, resembling Ni-terminated bimetallic surfaces that were predicted to be more active than Pt from theoretical and experimental studies on model surfaces. C1 [Tupy, Sarah A.; Bagia, Christina; Deng, Weihua; Huang, Yulin; Vlachos, Dionisios G.; Chen, Jingguang G.] Univ Delaware, Dept Chem & Bimol Engn, Catalysis Ctr Energy Innovat, Newark, DE 19716 USA. [Karim, Ayman M.] Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99352 USA. RP Vlachos, DG (reprint author), Univ Delaware, Dept Chem & Bimol Engn, Catalysis Ctr Energy Innovat, Newark, DE 19716 USA. EM vlachos@udel.edu; jgchen@udel.edu RI Karim, Ayman/G-6176-2012; OI Karim, Ayman/0000-0001-7449-542X; Vlachos, Dionisios/0000-0002-6795-8403 FU Catalysis Center for Energy Innovation, an Energy Frontier Research Center; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001004]; U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy; National Advanced Biofuels Consortium; Department of Energy's Office of Biomass Program; US Department of Energy, Office of Basic Energy Sciences [DE-FG02-05ER15688] FX The University of Delaware authors acknowledge support from the Catalysis Center for Energy Innovation, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award No. DE-SC0001004. The Pacific Northwest National Laboratory author acknowledges support from the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy and from the National Advanced Biofuels Consortium, which is funded by the Department of Energy's Office of Biomass Program with recovery act funds. Use of the National Synchrotron Light Source, Brookhaven National Laboratory, for the EXAFS experiments was supported by the US Department of Energy, Office of Basic Energy Sciences (Grant No. DE-FG02-05ER15688). SAT, is grateful to Prof. George W. Huber and Dr. Tushar Vispute for APR training and Vassili S. Vorotnikov for useful discussions. NR 42 TC 31 Z9 32 U1 6 U2 81 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2155-5435 J9 ACS CATAL JI ACS Catal. PD NOV PY 2012 VL 2 IS 11 BP 2290 EP 2296 DI 10.1021/cs3004227 PG 7 WC Chemistry, Physical SC Chemistry GA 032MT UT WOS:000310723900010 ER PT J AU Zhang, CJ Grass, ME Yu, Y Gaskell, KJ DeCaluwe, SC Chang, R Jackson, GS Hussain, Z Bluhm, H Eichhorn, BW Liu, Z AF Zhang, Chunjuan Grass, Michael E. Yu, Yi Gaskell, Karen J. DeCaluwe, Steven C. Chang, Rui Jackson, Gregory S. Hussain, Zahid Bluhm, Hendrik Eichhorn, Bryan W. Liu, Zhi TI Multielement Activity Mapping and Potential Mapping in Solid Oxide Electrochemical Cells through the use of operando XPS SO ACS CATALYSIS LA English DT Article DE ambient pressure XPS; ceria; solid oxide electrochemical cell; operando ID IN-SITU RAMAN; FUEL-CELLS; PHOTOELECTRON-SPECTROSCOPY; CARBON CORROSION; CERIA; OXIDATION; SURFACES; WATER AB Spatially resolved ambient pressure X-ray photoelectron spectroscopy has been used to measure and Visualize regions of electrochemical activity, local surface potential losses, overpotentials, and oxidation state changes on single sided ceria/yttria-stabilized zirconia (YSZ)/Pt solid oxide electrochemical cells. When hydrogen electro-oxidation (negative applied bias) or water electrolysis (positive applied bias) is promoted on the ceria electrocatalyst, the Ce3+/Ce4+ ratios shift away from equilibrium values and thereby demarcate electrochemically active regions on the ceria electrode. In addition to the ceria oxidation state shifts, inactive surface impurities with high photoelectron cross sections, such as Si, can provide local markers of activity through chemical and surface potential mappings under various electrochemical conditions. Localized removal of chemically active carbonaceous surface impurities also reveals regions of electrochemical oxidation activity on the ceria electrode. Finally, show that electrochemical polarization of solid oxide electrochemical cells under different gas environments is used to control the ceria surface Chemical state and oxygen vacancy density. C1 [DeCaluwe, Steven C.; Jackson, Gregory S.] Univ Maryland, Dept Mech Engn, College Pk, MD 20742 USA. [Zhang, Chunjuan; Yu, Yi; Gaskell, Karen J.; Eichhorn, Bryan W.] Univ Maryland, Dept Chem & Biochem, College Pk, MD 20742 USA. [Grass, Michael E.; Chang, Rui; Hussain, Zahid; Liu, Zhi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Bluhm, Hendrik] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Jackson, GS (reprint author), Univ Maryland, Dept Mech Engn, College Pk, MD 20742 USA. EM gsjackso@umd.edu; eichhorn@umd.edu; zliu2@lbl.gov RI Gaskell, Karen/H-8270-2014; Liu, Zhi/B-3642-2009; Jackson, Gregory/N-9919-2014 OI Liu, Zhi/0000-0002-8973-6561; Jackson, Gregory/0000-0002-8928-2459 FU Office of Naval Research [N000140510711]; University of Maryland Nanocenter; University of Maryland Energy Research Center (UMERC); Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was funded through the support of the Office of Naval Research through Contract No. N000140510711 (Dr. Michele Anderson program manager). We thank the University of Maryland Nanocenter and the University of Maryland Energy Research Center (UMERC) for support. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 30 TC 26 Z9 26 U1 7 U2 112 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2155-5435 J9 ACS CATAL JI ACS Catal. PD NOV PY 2012 VL 2 IS 11 BP 2297 EP 2304 DI 10.1021/cs3004243 PG 8 WC Chemistry, Physical SC Chemistry GA 032MT UT WOS:000310723900011 ER PT J AU Lobo, R Marshall, CL Dietrich, PJ Ribeiro, FH Akatay, C Stach, EA Mane, A Lei, Y Elam, J Miller, JT AF Lobo, Rodrigo Marshall, Christopher L. Dietrich, Paul J. Ribeiro, Fabio H. Akatay, Cem Stach, Eric A. Mane, Anil Lei, Yu Elam, Jeffrey Miller, Jeffrey T. TI Understanding the Chemistry of H-2 Production for 1-Propanol Reforming: Pathway and Support Modification Effects SO ACS CATALYSIS LA English DT Article DE biomass; Pt catalysts; liquid phase reforming; EXAFS; XANES ID RAY-ABSORPTION SPECTROSCOPY; HYDROGEN-PRODUCTION; GLYCEROL; CATALYSTS; BIOMASS; WATER; REACTOR; FUELS; HYDROCARBONS; OXYGEN AB The liquid-phase reforming of 1-propanol over a platinum-based catalyst on a number of supports was investigated. Propanol is being used as a surrogate for biomass-derived glycerol as a source of hydrogen in the conversion of cellulose to transportation fuels. The test conditions were high temperature (230-260 degrees C) and pressure (69 bar) in the presence of liquid water. Under these conditions, Pt over alumina coated (via atomic layer deposition) with a layer of approximately 1 nm of Al2O3, TiO2, or Ce2O3 (Pt-Al, Pt-Ti, Pt-Ce) is active for the reforming of 1-propariol. The Pt-Ti catalyst had the highest 1-propanol conversion rate per gram of catalyst followed by the Pt-Al and Pt-Ce catalysts, which had similar rates of reaction. Selectivity for each catalyst was primarily to ethane and CO, with the ratio between the two products being close to unity regardless of temperature., The hydrogen yield was constantly higher than twice the ethane yield, indicating that H-2 formation occurs before ethane is formed. Decarbonylation of propanal did not appear to contribute significantly to the formation of ethane. The propionic acid, which can produce: ethane and CO2 through decarboxylation,,is believed to form from the disproportionation of propanal. In contrast to the Canizzarro reaction, this reaction appears to be catalyzed by the supported Pt and not the support or in solution (through base Catalysis). Our analyses also showed that well dispersed Pt sinters under the high temperature and high partial pressure of Water in the reactor, and under reaction conditions that the surface of the Pt has high concentrations of CO (43% of the coverage of CO at room temperature) and water (96% of the coverage of water at 230 degrees C and 34 bar). C1 [Lobo, Rodrigo; Marshall, Christopher L.; Miller, Jeffrey T.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Mane, Anil; Lei, Yu; Elam, Jeffrey] Argonne Natl Lab, Div Energy Syst, Argonne, IL 60439 USA. [Dietrich, Paul J.; Ribeiro, Fabio H.; Akatay, Cem] Purdue Univ, Sch Chem Engn, W Lafayette, IN 47907 USA. [Stach, Eric A.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Marshall, CL (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM marshall@anl.gov RI Stach, Eric/D-8545-2011; ID, MRCAT/G-7586-2011; Marshall, Christopher/D-1493-2015; OI Stach, Eric/0000-0002-3366-2153; Marshall, Christopher/0000-0002-1285-7648; Lei, Yu/0000-0002-4161-5568; Ribeiro, Fabio/0000-0001-7752-461X FU Institute for Atom-efficient Chemical Transformations (IACT), an Energy Frontier Research Center; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences; U.S. Department of Energy Office of Science [DE-AC02-06CH11357]; U.S. DOE [DE-AC02-06CH11357] FX This material is based upon work supported as part of the Institute for Atom-efficient Chemical Transformations (IACT), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. Argonne National Laboratory, a U.S. Department of Energy Office of Science laboratory, is operated under Contract No. DE-AC02-06CH11357.; Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. MRCAT operations are supported by the Department of Energy and the MRCAT member institutions. NR 30 TC 14 Z9 14 U1 3 U2 59 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2155-5435 J9 ACS CATAL JI ACS Catal. PD NOV PY 2012 VL 2 IS 11 BP 2316 EP 2326 DI 10.1021/cs300405s PG 11 WC Chemistry, Physical SC Chemistry GA 032MT UT WOS:000310723900013 ER PT J AU Benavidez, AD Kovarik, L Genc, A Agrawal, N Larsson, EM Hansen, TW Karim, AM Datye, AK AF Benavidez, Angelica D. Kovarik, Libor Genc, Arda Agrawal, Nitin Larsson, Elin M. Hansen, Thomas W. Karim, Ayman M. Datye, Abhaya K. TI Environmental Transmission Electron Microscopy Study of the Origins of Anomalous Particle Size Distributions in Supported Metal Catalysts SO ACS CATALYSIS LA English DT Article DE catalyst sintering; Ostwald ripening particle size distributions; Pt/SiO2; Pd/carbon; environmental TEM ID HETEROGENEOUS CATALYSTS; GROWTH; NANOPARTICLES; COALESCENCE; BEHAVIOR; ISLANDS; SURFACE AB In this Environmental Transmission Electron Microscopy (ETEM) study we examined the growth patterns' of uniform distributions of nanoparticles (NPs) using model catalysts. Pt/SiO2 was heated at 550 degrees C in 560 Pa of O-2 while Pd/carbon was heated in vacuum at 500 degrees C and in 300 Pa of 5%H-2 in Argon at temperatures up to 600 degrees C. Individual NPs of Pd were tracked to determine the operative sintering mechanisms. We found anomalous growth Of NPs occurred during the early stages of catalyst sintering wherein some particles started to grow significantly larger than the mean, resulting in a broadening of the particle size distribution (PSD). The abundance of the larger particles did not fit the log normal distribution. We can rule out sample nonuniformity as a cause for the growth of these large particles, since images were recorded prior to heat treatments. The anomalous growth of these particles may help explain PSDs in heterogeneous catalysts which often show particles that are significantly larger than the mean, resulting in a long tail to the right. It has been suggested previously that particle migration and coalescence could be the likely cause for such broad size distributions. We did not detect any random migration of the NPs leading to coalescence. A directed migration process was seen to occur at elevated temperatures for Pd/carbon under H-2. This study shows that anomalous growth of NPs can occur under conditions where Ostwald ripening is the primary sintering mechanism. C1 [Hansen, Thomas W.] Tech Univ Denmark, Ctr Electron Nanoscopy, DK-2800 Lyngby, Denmark. [Benavidez, Angelica D.; Datye, Abhaya K.] Univ New Mexico, Dept Chem & Nucl Engn, Albuquerque, NM 87131 USA. [Benavidez, Angelica D.; Datye, Abhaya K.] Univ New Mexico, Ctr Microengn Mat, Albuquerque, NM 87131 USA. [Kovarik, Libor] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Kovarik, Libor; Agrawal, Nitin; Karim, Ayman M.] Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99352 USA. [Genc, Arda] FEI Co, USA NanoPort, Hillsboro, OR 97124 USA. [Larsson, Elin M.] Chalmers, Dept Appl Phys, Div Phys Chem, S-41296 Gothenburg, Sweden. [Larsson, Elin M.] Chalmers, Competence Ctr Catalysis, S-41296 Gothenburg, Sweden. RP Hansen, TW (reprint author), Tech Univ Denmark, Ctr Electron Nanoscopy, DK-2800 Lyngby, Denmark. EM thomas.w.hansen@cen.dtu.dk; Ayman.Karim@pnnl.gov; datye@unm.edu RI Karim, Ayman/G-6176-2012; Hansen, Thomas/H-5367-2011; Kovarik, Libor/L-7139-2016; OI Karim, Ayman/0000-0001-7449-542X; Hansen, Thomas/0000-0002-1861-3054; Datye, Abhaya/0000-0002-7126-8659 FU Chemical Imaging Initiative at Pacific Northwest National Laboratory (PNNL); National Science Foundation's GRFP under NSF [DGE-0237002 G]; NSF [OISE 0730277]; DOE [DE-FG02-05ER15712]; PNNL through the Chemical Imaging Initiative FX The research described in this paper was supported, in part, by the Chemical Imaging Initiative at Pacific Northwest National Laboratory (PNNL). It was conducted under the Laboratory Directed Research and Development Program at PNNL, a multi program national laboratory operated by Battelle for the U.S. Department of Energy. A.D.B. acknowledges the National Science Foundation's GRFP under NSF Grant DGE-0237002 G. A.K.D. and A.D.B. acknowledge financial support from NSF Grant OISE 0730277, DOE Grant DE-FG02-05ER15712, and a contract from PNNL through the Chemical Imaging Initiative. The A. P. Moller and Chastine Mc-Kinney Moller Foundation is gratefully acknowledged for its contribution towards the establishment of the Center for Electron Nanoscopy in the Technical University of Denmark where the Pt ETEM experiments were performed. The Pd ETEM experiments were performed at the Environmental Molecular Sciences Laboratory (EMSL), a user facility operated by the DOE at PNNL. NR 27 TC 23 Z9 23 U1 6 U2 80 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2155-5435 J9 ACS CATAL JI ACS Catal. PD NOV PY 2012 VL 2 IS 11 BP 2349 EP 2356 DI 10.1021/cs3005117 PG 8 WC Chemistry, Physical SC Chemistry GA 032MT UT WOS:000310723900016 ER PT J AU Kweskin, SJ Rioux, RM Song, H Komvopoulos, K Yang, P Somorjai, GA AF Kweskin, S. J. Rioux, R. M. Song, H. Komvopoulos, K. Yang, P. Somorjai, G. A. TI High-Pressure Adsorption of Ethylene on Cubic Pt Nanoparticles and Pt(100) Single Crystals Probed by in Situ Sum Frequency Generation Vibrational Spectroscopy SO ACS CATALYSIS LA English DT Article DE adsorbate-induced reconstruction; carbon monoxide; ethylene; nanoparticles; platinum; single crystals; sum-frequency generation (SFG) vibrational spectroscopy; poly(vinylpyrrolidone) ID NONLINEAR-OPTICAL SPECTROSCOPY; PLATINUM NANOPARTICLES; CATALYTIC-REACTIONS; STRUCTURE SENSITIVITY; ATMOSPHERIC-PRESSURE; METAL NANOPARTICLES; MODEL CATALYSTS; THERMAL-DECOMPOSITION; NANOCLUSTER FORMATION; GOLD NANOPARTICLES AB A model catalytic system of a monolayer consisting of 9-nm average size, cubic, single crystal Pt nanoparticles and poly,(vinylpyrrolidone) (PVP) polymer capping agent deposited on a sapphire prism was investigated by sum-frequency generation (SFG) vibrational spectroscopy in total internal reflection (TIR) geometry. Exposure of a clean nanoparticle monolayer after removal of PVP,by cyclic oxidation-reduction treatment to high-pressure ethylene at room temperature led to the formation of ethylidyne and di-sigma bonded ethylene. Low-pressure ethylene adsorption on a pseudohexagonal reconstructed Pt(100) single crystal resulted only in the formation of di-sigma bonded ethylene. High-pressure adsorption of ethylene on Pt nanoparticle monolayers and Pt(100) led to the formation of both ethylidyne and di-sigma bonded ethylene and stabilized the pseudohexagonal reconstruction of Pt(100) On both the single crystal and the surface of clean cubic nanoparticles. Restructuring of the PVP layer caused by CO adsorption indicated a small fraction of the Pt surface was available for adsorption. The stretching frequency of linear bound CO red shifted relative to CO adsorption on a clean Pt nanoparticle monolayer. PVP reversibly restructured upon the removal of CO by oxidation at room temperature. After the near complete removal of PVP by a cyclic low-temperature oxidation reduction process, the peak position of the linear-bound CO blue-shifted to a frequency consistent with the adsorption of CO on a clean Pt surface. The successful application of TIR-SFG to catalytically relevant surfaces under high-pressure conditions demonstrated in this study is a significant advance in the detection of surface intermediates. C1 [Kweskin, S. J.; Rioux, R. M.; Song, H.; Yang, P.; Somorjai, G. A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Komvopoulos, K.] Univ Calif Berkeley, Dept Mech Engn, Berkeley, CA 94720 USA. [Kweskin, S. J.; Rioux, R. M.; Song, H.; Yang, P.; Somorjai, G. A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Rioux, RM (reprint author), Penn State Univ, Dept Chem Engn, University Pk, PA 16802 USA. EM rioux@engr.psu.edu; somorjai@berkeley.edu RI Song, Hyunjoon/C-1638-2011 OI Song, Hyunjoon/0000-0002-1565-5697 FU Office of Science, Office of Advanced Scientific Computing Research, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U.S. Department of Energy [DE-AC02-05CH11231]; Ford Motor Company FX This work was supported by the Director, Office of Science, Office of Advanced Scientific Computing Research, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. R.M.R. would like to acknowledge Ford Motor Company for financial support through a graduate fellowship administered by the Berkeley Catalysis Center. NR 87 TC 11 Z9 11 U1 6 U2 71 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2155-5435 J9 ACS CATAL JI ACS Catal. PD NOV PY 2012 VL 2 IS 11 BP 2377 EP 2386 DI 10.1021/cs3005067 PG 10 WC Chemistry, Physical SC Chemistry GA 032MT UT WOS:000310723900019 ER PT J AU Karim, AM Howard, C Roberts, B Kovarik, L Zhang, L King, DL Wang, Y AF Karim, Ayman M. Howard, Christopher Roberts, Benjamin Kovarik, Libor Zhang, Liang King, David L. Wang, Yong TI In Situ X-ray Absorption Fine Structure Studies on the Effect of pH on Pt Electronic Density during Aqueous Phase Reforming of Glycerol SO ACS CATALYSIS LA English DT Article DE In situ EXAFS; XANES; Pt/C; pH; aqueous phase reforming; adsorbates; electronic density ID FAST PYROLYSIS PROCESSES; TRANSPORTATION FUELS; CATALYTIC CONVERSION; BIOMASS; HYDROCARBONS; SPECTROSCOPY; SPECTRA; ALKANES; CARBON; EXAFS AB In situ X-ray absorption spectroscopy (XAS) results on correlating the Pt local coordination and electronic structure with the Pt/C catalyst activity and selectivity during aqueous reforming of glycerol at different pH are reported. The results show that both low and high pH favor C-O cleavage over that of C-C. However, the selectivity toward C-O bond cleavage was higher under the acidic conditions. XANES measurements under reaction conditions showed that low pH increased the Pt electron density while the effect of basic conditions was minimal. Delta XANES was used to estimate the coverage of adsorbates under reaction conditions and the results suggest a change in the adsorbates coverage by the acidic conditions, resulting in higher electron density on Pt. C1 [Karim, Ayman M.; Howard, Christopher; Roberts, Benjamin; Kovarik, Libor; Zhang, Liang; King, David L.; Wang, Yong] Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99352 USA. [Kovarik, Libor] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Wang, Yong] Washington State Univ, Dept Chem Engn, Pullman, WA 99164 USA. RP Karim, AM (reprint author), Pacific NW Natl Lab, Inst Integrated Catalysis, POB 999, Richland, WA 99352 USA. EM ayman.karim@pnnl.gov RI Wang, Yong/C-2344-2013; Karim, Ayman/G-6176-2012; Kovarik, Libor/L-7139-2016 OI Karim, Ayman/0000-0001-7449-542X; FU U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy; National Advanced Biofuels Consortium; Department of Energy's Office of Biomass Program; U.S. Department of Energy, Office of Basic Energy Sciences [DE-FG02-05ER15688] FX The authors acknowledge financial support from the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy and from the National Advanced Biofuels Consortium, which is funded by the Department of Energy's Office of Biomass Program with recovery act funds. The TEM experiments were carried out at the Environmental and Molecular Sciences Laboratory, a user facility of the Department of Energy, of the Pacific Northwest National Laboratory. Use of the National Synchrotron Light Source, Brookhaven National Laboratory, for the EXAFS experiments was supported by the U.S. Department of Energy, Office of Basic Energy Sciences (Grant DE-FG02-05ER15688). NR 28 TC 16 Z9 16 U1 1 U2 42 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2155-5435 J9 ACS CATAL JI ACS Catal. PD NOV PY 2012 VL 2 IS 11 BP 2387 EP 2394 DI 10.1021/cs3005049 PG 8 WC Chemistry, Physical SC Chemistry GA 032MT UT WOS:000310723900020 ER PT J AU Tyo, EC Yin, CR Di Vece, M Qian, Q Kwon, G Lee, S Lee, B DeBartolo, JE Seifert, S Winans, RE Si, R Ricks, B Goergen, S Rutter, M Zugic, B Flytzani-Stephanopoulos, M Wang, ZW Palmer, RE Neurock, M Vajda, S AF Tyo, Eric C. Yin, Chunrong Di Vece, Marcel Qian, Qiang Kwon, Gihan Lee, Sungsik Lee, Byeongdu DeBartolo, Janae E. Seifert, Soenke Winans, Randall E. Si, Rui Ricks, Brian Goergen, Simone Rutter, Matthew Zugic, Branko Flytzani-Stephanopoulos, Maria Wang, Zhi Wei Palmer, Richard E. Neurock, Matthew Vajda, Stefan TI Oxidative Dehydrogenation of Cyclohexane on Cobalt Oxide (Co3O4) Nanoparticles: The Effect of Particle Size on Activity and Selectivity SO ACS CATALYSIS LA English DT Article DE oxidative dehydrogenation; cyclohexane; cobalt oxide; Co3O4; size effect; in situ X-ray scattering; GISAXS; in situ X-ray absorption; GIXANES; temperature programmed reaction; transmission electron microscopy; scanning transmission electron microscopy; X-ray diffraction; mass spectrometry; assembly; density functional theory; alkane activation; alkene activation ID INITIO MOLECULAR-DYNAMICS; CHEMICAL-VAPOR-DEPOSITION; FISCHER-TROPSCH SYNTHESIS; TRANSITION-METAL OXIDES; AUGMENTED-WAVE METHOD; H BOND ACTIVATION; IN-SITU GISAXS; PLATINUM CLUSTERS; THIN-FILMS; HYDROGEN-PRODUCTION AB The oxidative dehydrogenation of cyclohexane by cobalt oxide nanoparticles was studied via temperature programmed reaction combined with in situ grazing incidence X-ray absorption spectroscopy and grazing incidence small-angle X-ray scattering and theoretical calculations on model Co3O4 substrates. Both 6 and 12 nm Co3O4 nanoparticles were made through a surfactant-free preparation and dispersed on an Al2O3 surface formed by atomic layer deposition. Under reaction conditions the nanoparticles retained their oxidation state and did. not sinter. They,instead underwent an assembly/disassembly process and could reorganize within their assemblies. The selectivity of the catalyst was found to be size- and temperature dependent, with larger particles preferentially producing cyclohexene at lower temperatures and smaller particles predominantly resulting in benzene at higher temperatures. The mechanistic features thought to control the oxidative dehydrogenation of cyclohexane and other light alkanes on cobalt oxide were established by carrying out density functional theory calculations on the activation of propane, a surrogate model alkane, over model Co3O4 surfaces. The initial activation of the alkane. (propane) proceeds via hydrogen abstraction over surface oxygen sites. The subsequent activation of the resulting alkoxide intermediate occurs at a second surface oxygen site to form the alkene (propene) which then desorbs from the surface. Hydroxyl recombination results in the formation of water which desorbs from the surface. Oxygen is necessary to regenerate the surface oxygen sites, catalyze C-H activation steps, and minimize catalyst degradation. C1 [Qian, Qiang; Neurock, Matthew] Univ Virginia, Dept Chem Engn, Charlottesville, VA 22904 USA. [Neurock, Matthew] Univ Virginia, Dept Chem, Charlottesville, VA 22904 USA. [Tyo, Eric C.; Di Vece, Marcel; Vajda, Stefan] Yale Univ, Sch Engn & Appl Sci, Dept Chem & Environm Engn, New Haven, CT 06520 USA. [Yin, Chunrong; Kwon, Gihan; Vajda, Stefan] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Lee, Sungsik; Lee, Byeongdu; DeBartolo, Janae E.; Seifert, Soenke; Winans, Randall E.] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. [Vajda, Stefan] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Si, Rui; Ricks, Brian; Goergen, Simone; Rutter, Matthew; Zugic, Branko; Flytzani-Stephanopoulos, Maria] Tufts Univ, Dept Chem & Biol Engn, Medford, MA 02155 USA. [Wang, Zhi Wei; Palmer, Richard E.] Univ Birmingham, Sch Phys & Astron, Nanoscale Phys Res Lab, Birmingham B15 2TT, W Midlands, England. RP Neurock, M (reprint author), Univ Virginia, Dept Chem Engn, 102 Engineers Way, Charlottesville, VA 22904 USA. EM mn4n@virginia.edu; vajda@anl.gov RI Yin, Chunrong/F-8802-2012; Palmer, Richard/A-5366-2008; Di Vece, Marcel/N-6957-2016; OI Palmer, Richard/0000-0001-8728-8083; Di Vece, Marcel/0000-0002-0041-4348; Lee, Byeongdu/0000-0003-2514-8805 FU MURI grant from the Air Force Office of Sponsored Research [FA9550-08-0309]; U.S. Department of Energy, BES Materials Sciences [DE-AC-02-06CH11357]; U.S. DOE [DE-AC02-06CH11357]; Department of Energy's Office of Biological and Environmental Research; UChicago Argonne, LLC FX We are grateful for the financial support to support this work at Virginia, Tufts, and Yale by a MURI grant from the Air Force Office of Sponsored Research FA9550-08-0309. The effort at Argonne (in situ data acquisition and analysis) was supported by the U.S. Department of Energy, BES Materials Sciences, under Contract DE-AC-02-06CH11357, with UChicago Argonne, LLC, operator of Argonne National Laboratory. The use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. The computational research was performed using EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. NR 100 TC 41 Z9 41 U1 15 U2 231 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2155-5435 J9 ACS CATAL JI ACS Catal. PD NOV PY 2012 VL 2 IS 11 BP 2409 EP 2423 DI 10.1021/cs300479a PG 15 WC Chemistry, Physical SC Chemistry GA 032MT UT WOS:000310723900023 ER PT J AU Allotta, PM Stair, PC AF Allotta, Paula M. Stair, Peter C. TI Time-Resolved Studies of Ethylene and Propylene Reactions in Zeolite H-MFI by In-Situ Fast IR Heating and UV Raman Spectroscopy SO ACS CATALYSIS LA English DT Article DE ethylene; propylene; UV-Raman; coke; zeolite; H-MFI ID TO-GASOLINE CHEMISTRY; COKE FORMATION; REACTION-MECHANISM; HYDROCARBON FORMATION; MOLECULAR-DYNAMICS; ACIDIC ZEOLITES; CARBENIUM ION; METHANOL; CONVERSION; PROPENE AB The conversion of ethylene and propylene absorbed in zeolite H-MFI was studied using UV Raman spectroscopy. To observe early stage reaction intermediates, an infrared laser was used as a fast heating source. Alkyl substituted naphthalenes and fluorenes, which have been previously suggested as hydrocarbon pool species, were observed regardless of the olefin reagent. Conjugated dienes were formed from propylene but not observed for ethylene at short reaction times. Conventional heating in a furnace was used to force the reaction to completion. For propylene sheet like polyaromatic hydrocarbons were formed immediately. For ethylene cyclic dienes, conjugated olefins, and ultimately sheet like polyaromatic hydrocarbons were formed at progressively higher reaction temperatures. The results show that the polyaromatic species implicated as deactivating coke in zeolite catalysts can be formed by conversion of polyenes. C1 [Allotta, Paula M.; Stair, Peter C.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Stair, Peter C.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Stair, PC (reprint author), Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. EM pstair@northwestern.edu FU Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy [DE-FG02-97ER14789] FX Financial support of this work was provided by the Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy under Grant DE-FG02-97ER14789. NR 49 TC 5 Z9 5 U1 5 U2 73 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2155-5435 J9 ACS CATAL JI ACS Catal. PD NOV PY 2012 VL 2 IS 11 BP 2424 EP 2432 DI 10.1021/cs3004215 PG 9 WC Chemistry, Physical SC Chemistry GA 032MT UT WOS:000310723900024 ER PT J AU Wu, TP Childers, DJ Gomez, C Karim, AM Schweitzer, NM Kropf, AJ Wang, H Bolin, TB Hu, YF Kovarik, L Meyer, RJ Miller, JT AF Wu, Tianpin Childers, David J. Gomez, Carolina Karim, Ayman M. Schweitzer, Neil M. Kropf, A. Jeremy Wang, Hui Bolin, Trudy B. Hu, Yongfeng Kovarik, Libor Meyer, Randall J. Miller, Jeffrey T. TI General Method for Determination of the Surface Composition in Bimetallic Nanoparticle Catalysts from the L Edge X-ray Absorption Near-Edge Spectra SO ACS CATALYSIS LA English DT Article DE PtPd bimetallic catalysts; neopentane hydrogenolysis and isomerization; bimetallic nanoparticle surface composition; L edge XANES of Pt; L edge XANES of Pd ID TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; CARBON-MONOXIDE; PARTICLE-SIZE; SELECTIVE HYDROGENATION; PT-SN/AL2O3 CATALYSTS; PT-AU/SIO2 CATALYSTS; CHEMICAL-PROPERTIES; OXYGEN REDUCTION; CO ADSORPTION AB Bimetallic PtPd on silica nanoparticle catalysts have been synthesized, and their average structure has been determined by Pt L-3 and Pd K edge extended X-ray absorption fine structure spectroscopy. The bimetallic structure is confirmed from elemental line scans by scanning transmission electron microscopy of the individual 2-nm-sized particles. A general method is described to determine the surface composition of bimetallic nanoparticles even when both metals adsorb; for example, CO, by combining the quantitative characterization by X-ray absorption near-edge structure spectra at L edges with CO adsorption with the adsorption stoichiometry determined by Fourier transform infrared spectroscopy. Determination of the surface composition leads to a better understanding of the changes in catalytic chemistry that accompany alloy formation. Although monometallic Pt and Pd have similar turnover rates for neopentane hydrogenolysis and isomerization, on the basis of the surface composition, it appears that in the bimetallic PtPd catalysts, the rate and products are determined predominantly by Pt with little contribution from surface Pd. Density functional theory calculations indicate that the center of the Pt d-band density of states shifts to higher energy, or closer to the Fermi level, whereas that in Pd shifts to lower energy away from the Fermi level. Similarly, the calculated enthalpy of CO adsorption increases on Pt, but decreases on Pd. It is speculated that because of the very low surface coverage of the neopentane reaction intermediates, only surface atoms that form the strongest bonds are catalytically active-that is, Pt-rather than all surface atoms. The dominant role of Pd, therefore, appears to be to (slightly) modify Pt rather than to contribute to the catalytic conversion. C1 [Childers, David J.; Gomez, Carolina; Meyer, Randall J.] Univ Illinois, Dept Chem Engn, Chicago, IL 60612 USA. [Bolin, Trudy B.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Wu, Tianpin; Schweitzer, Neil M.; Kropf, A. Jeremy; Miller, Jeffrey T.] Argonne Natl Lab, Div Chem Sci & Engn, Argonne, IL 60439 USA. [Karim, Ayman M.; Kovarik, Libor] Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99352 USA. [Wang, Hui] Univ Saskatchewan, Dept Chem & Biol Engn, Saskatoon, SK S7N 5A2, Canada. [Hu, Yongfeng] Canadian Light Source, Saskatoon, SK S7N 0X4, Canada. RP Meyer, RJ (reprint author), Univ Illinois, Dept Chem Engn, Chicago, IL 60612 USA. EM rjm@uic.edu; millerjt@anl.gov RI BM, MRCAT/G-7576-2011; ID, MRCAT/G-7586-2011; Karim, Ayman/G-6176-2012; Kovarik, Libor/L-7139-2016 OI Karim, Ayman/0000-0001-7449-542X; FU Institute for Atom-Efficient Chemical Transformations (IACT), an Energy Frontier Research Center; National Science Foundation (CBET) [0747646]; U.S. Department of Energy's Office of Biological and Environmental Research; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; National Advanced Biofuels Consortium; Department of Energy's Office of Biomass Program; U.S. DOE [DE-AC02-06CH11357] FX This material is based upon work supported as part of the Institute for Atom-Efficient Chemical Transformations (IACT), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. R.J.M., C.G., and D.C. gratefully acknowledge funding for this work from the National Science Foundation (CBET Grant No. 0747646). We gratefully acknowledge LCRC at Argonne National Lab for allocation grant intermetallic, which was used to perform most of the calculations described herein. The STEM and EDS work was performed in the Environmental Molecular Sciences Laboratory, a national scientific user facility sponsored by the U.S. Department of Energy's Office of Biological and Environmental Research, located at Pacific Northwest National Laboratory (PNNL) in Richland, WA. Use of the Center for Nanoscale Materials was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. The work was supported by the National Advanced Biofuels Consortium, which is funded by the Department of Energy's Office of Biomass Program with recovery act funds. Use of the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. MRCAT operations are supported by the Department of Energy and the MRCAT member institutions. Use of the 9 muB beamline at the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. NR 74 TC 9 Z9 9 U1 4 U2 65 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2155-5435 J9 ACS CATAL JI ACS Catal. PD NOV PY 2012 VL 2 IS 11 BP 2433 EP 2443 DI 10.1021/cs3004566 PG 11 WC Chemistry, Physical SC Chemistry GA 032MT UT WOS:000310723900025 ER PT J AU Hoke, ET Sachs-Quintana, IT Lloyd, MT Kauvar, I Mateker, WR Nardes, AM Peters, CH Kopidakis, N McGehee, MD AF Hoke, Eric T. Sachs-Quintana, I. T. Lloyd, Matthew T. Kauvar, Isaac Mateker, William R. Nardes, Alexandre M. Peters, Craig H. Kopidakis, Nikos McGehee, Michael D. TI The Role of Electron Affinity in Determining Whether Fullerenes Catalyze or Inhibit Photooxidation of Polymers for Solar Cells SO ADVANCED ENERGY MATERIALS LA English DT Article DE degradation; organic solar cells; photooxidation; photovoltaics; electron affinity ID CONJUGATED POLYMERS; SINGLET OXYGEN; MDMO-PPV; REACTIVE INTERMEDIATE; TRIPLET FORMATION; BLENDS; DEGRADATION; EFFICIENCY; ENERGY; PHOTODEGRADATION AB Understanding the stability and degradation mechanisms of organic solar materials is critically important to achieving long device lifetimes. Here, an investigation of the photodegradation of polymer:fullerene blend films exposed to ambient conditions for a variety of polymer and fullerene derivative combinations is presented. Despite the wide range in polymer stabilities to photodegradation, the rate of irreversible polymer photobleaching in blend films is found to consistently and dramatically increase with decreasing electron affinity of the fullerene derivative. Furthermore, blends containing fullerenes with the smallest electron affinities photobleached at a faster rate than films of the pure polymer. These observations can be explained by a mechanism where both the polymer and fullerene donate photogenerated electrons to diatomic oxygen to form the superoxide radical anion which degrades the polymer. C1 [Hoke, Eric T.; Sachs-Quintana, I. T.; Kauvar, Isaac; Mateker, William R.; Peters, Craig H.; McGehee, Michael D.] Stanford Univ, Dept Mat Sci & Engn, Stanford, CA 94305 USA. [Lloyd, Matthew T.; Nardes, Alexandre M.; Kopidakis, Nikos] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP McGehee, MD (reprint author), Stanford Univ, Dept Mat Sci & Engn, 476 Lomita Mall, Stanford, CA 94305 USA. EM mmcgehee@stanford.edu RI Nardes, Alexandre/C-8556-2012; Kopidakis, Nikos/N-4777-2015 FU Center for Advanced Molecular Photovoltaics, King Abdullah University of Science and Technology (KAUST) [KUS-C1-015-21]; US Department of Energy [DE-AC36-08-GO28308]; National Renewable Energy Laboratory through the DOE SETP program; Fannie and John Hertz Foundation; National Science Foundation; DOE SULI fellowship program FX E.T.H., I.T.S.Q., and M.T.L. contributed equally to this work. This publication was supported by the Center for Advanced Molecular Photovoltaics (Award No KUS-C1-015-21), made by King Abdullah University of Science and Technology (KAUST). M.T.L, A.M.N and N.K. acknowledge support from the US Department of Energy under Contract No. DE-AC36-08-GO28308 with the National Renewable Energy Laboratory through the DOE SETP program. We thank Plextronics for providing some of the fullerenes (ICMA, ICBA, and ICTA) and LG providing the sulfur plasma lamps. We thank H.-J. Egelhaaf for helpful discussions. Additional support was provided for E.T.H. by the Fannie and John Hertz Foundation, for I.T.S.Q. by the National Science Foundation Graduate Research Fellowship and I. K. was supported by the DOE SULI fellowship program. NR 43 TC 66 Z9 66 U1 3 U2 74 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1614-6832 J9 ADV ENERGY MATER JI Adv. Energy Mater. PD NOV PY 2012 VL 2 IS 11 BP 1351 EP 1357 DI 10.1002/aenm.201200169 PG 7 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Energy & Fuels; Materials Science; Physics GA 031YJ UT WOS:000310678300009 ER PT J AU Brushett, FR Vaughey, JT Jansen, AN AF Brushett, Fikile R. Vaughey, John T. Jansen, Andrew N. TI An All-Organic Non-aqueous Lithium-Ion Redox Flow Battery SO ADVANCED ENERGY MATERIALS LA English DT Article DE redox-active organic molecules; energy storage; redox flow batteries; quinoxaline; lithium-ions ID ELECTROCHEMICAL OVERCHARGE PROTECTION; CELLS; ADDITIVES; SHUTTLES AB A non-aqueous lithium-ion redox flow battery employing organic molecules is proposed and investigated. 2,5-Di-tert-butyl-1,4-bis(2-methoxyethoxy)benzene and a variety of molecules derived from quinoxaline are employed as initial high-potential and low-potential active materials, respectively. Electrochemical measurements highlight that the choice of electrolyte and of substituent groups can have a significant impact on redox species performance. The charge-discharge characteristics are investigated in a modified coin-cell configuration. After an initial break-in period, coulombic and energy efficiencies for this unoptimized system are similar to 70% and similar to 37%, respectively, with major charge and discharge plateaus between 1.8-2.4 V and 1.7-1.3 V, respectively, for 30 cycles. Performance enhancements are expected with improvements in cell design and materials processing. C1 [Brushett, Fikile R.; Vaughey, John T.; Jansen, Andrew N.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Jansen, AN (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM jansen@anl.gov RI Jansen, Andrew/Q-5912-2016; OI Jansen, Andrew/0000-0003-3244-7790; Vaughey, John/0000-0002-2556-6129 FU US Department of Energy, Office of Science [DE-AC02-06CH11357]; Argonne National Laboratory FX This work was supported by the US Department of Energy, Office of Science, under Contract DE-AC02-06CH11357. F.R.B. is supported by a Director's Postdoctoral Fellowship at Argonne National Laboratory. We thank Lu Zhang, Zhengcheng Zhang, Chris Johnson, Zonghai Chen, Mike Slater, and Susanna Neuhold for stimulating discussion. We also appreciate the experimental support of Bryant Polzin and Lynn Trahey, as well as Greg Krumdick and the staff of the Materials Engineering Research Facility at Argonne National Laboratory. NR 29 TC 114 Z9 114 U1 21 U2 244 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1614-6832 J9 ADV ENERGY MATER JI Adv. Energy Mater. PD NOV PY 2012 VL 2 IS 11 BP 1390 EP 1396 DI 10.1002/aenm.201200322 PG 7 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Energy & Fuels; Materials Science; Physics GA 031YJ UT WOS:000310678300014 ER PT J AU Dominik, M Belczynski, K Fryer, C Holz, DE Berti, E Bulik, T Mandel, I O'Shaughnessy, R AF Dominik, Michal Belczynski, Krzysztof Fryer, Christopher Holz, Daniel E. Berti, Emanuele Bulik, Tomasz Mandel, Ilya O'Shaughnessy, Richard TI DOUBLE COMPACT OBJECTS. I. THE SIGNIFICANCE OF THE COMMON ENVELOPE ON MERGER RATES SO ASTROPHYSICAL JOURNAL LA English DT Article DE binaries: general; black hole physics; stars: evolution; stars: neutron ID BLACK-HOLE BINARIES; GAMMA-RAY BURSTS; BINDING-ENERGY PARAMETER; MASSIVE CLOSE BINARIES; NEUTRON-STAR SYSTEMS; O-TYPE STARS; GLOBULAR-CLUSTERS; INSPIRALING BINARIES; EXPLOSION MECHANISM; GRAVITATIONAL-WAVES AB The last decade of observational and theoretical developments in stellar and binary evolution provides an opportunity to incorporate major improvements to the predictions from population synthesis models. We compute the Galactic merger rates for NS-NS, BH-NS, and BH-BH mergers with the StarTrack code. The most important revisions include updated wind mass-loss rates (allowing for stellar-mass black holes up to 80 M-circle dot), a realistic treatment of the common envelope phase (a process that can affect merger rates by 2-3 orders of magnitude), and a qualitatively new neutron star/black hole mass distribution (consistent with the observed "mass gap"). Our findings include the following. (1) The binding energy of the envelope plays a pivotal role in determining whether a binary merges within a Hubble time. (2) Our description of natal kicks from supernovae plays an important role, especially for the formation of BH-BH systems. (3) The masses of BH-BH systems can be substantially increased in the case of low metallicities or weak winds. (4) Certain combinations of parameters underpredict the Galactic NS-NS merger rate and can be ruled out. (5) Models incorporating delayed supernovae do not agree with the observed NS/BH "mass gap," in accordance with our previous work. This is the first in a series of three papers. The second paper will study the merger rates of double compact objects as a function of redshift, star formation rate, and metallicity. In the third paper, we will present the detection rates for gravitational-wave observatories, using up-to-date signal waveforms and sensitivity curves. C1 [Dominik, Michal; Belczynski, Krzysztof; Bulik, Tomasz] Univ Warsaw, Astron Observ, PL-00478 Warsaw, Poland. [Belczynski, Krzysztof] Univ Texas Brownsville, Ctr Gravitat Wave Astron, Brownsville, TX 78520 USA. [Holz, Daniel E.] Univ Chicago, Enrico Fermi Inst, Dept Phys, Chicago, IL 60637 USA. [Holz, Daniel E.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Holz, Daniel E.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Berti, Emanuele] Univ Mississippi, Dept Phys & Astron, University, MS 38677 USA. [Berti, Emanuele] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Mandel, Ilya] Univ Birmingham, Sch Phys & Astron, Birmingham B15 2TT, W Midlands, England. [O'Shaughnessy, Richard] Univ Wisconsin, Ctr Gravitat & Cosmol, Milwaukee, WI 53211 USA. RP Dominik, M (reprint author), Univ Warsaw, Astron Observ, Al Ujazdowskie 4, PL-00478 Warsaw, Poland. RI Berti, Emanuele/C-9331-2016; OI Berti, Emanuele/0000-0003-0751-5130; O'Shaughnessy, Richard/0000-0001-5832-8517; Mandel, Ilya/0000-0002-6134-8946 FU National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396]; NSF [PHY-0900735, PHY-1055103, PHY-0970074]; Bradley Program Fellowship; UWM Research Growth Initiative; Polish grant [N N203 511238, DPN/N176/VIRGO/2009, N N203 302835, GR-4071] FX We thank Francesca Valsecchi for providing detailed calculations of specific mass transfer scenarios. We also thank the N. Copernicus Astronomical Centre in Warsaw, Poland, and the University of Texas at Brownsville, USA, for their courtesy in allowing us to use their computational resources. Work at LANL was done under the auspices of the National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396. E.B. is supported by NSF grant PHY-0900735 and by NSF CAREER grant PHY-1055103. R.O.S. is currently supported by NSF award PHY-0970074, the Bradley Program Fellowship, and the UWM Research Growth Initiative. T.B. is supported by the Polish grants N N203 511238 and DPN/N176/VIRGO/2009. K.B. is supported by the Polish grant N N203 302835. M.D. is supported by the Polish grant GR-4071. NR 82 TC 148 Z9 148 U1 0 U2 5 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X J9 ASTROPHYS J JI Astrophys. J. PD NOV 1 PY 2012 VL 759 IS 1 AR 52 DI 10.1088/0004-637X/759/1/52 PG 28 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 030JL UT WOS:000310566900052 ER PT J AU Jordan, GC Graziani, C Fisher, RT Townsley, DM Meakin, C Weide, K Reid, LB Norris, J Hudson, R Lamb, DQ AF Jordan, G. C. Graziani, C. Fisher, R. T. Townsley, D. M. Meakin, C. Weide, K. Reid, L. B. Norris, J. Hudson, R. Lamb, D. Q. TI THE DETONATION MECHANISM OF THE PULSATIONALLY ASSISTED GRAVITATIONALLY CONFINED DETONATION MODEL OF Type Ia SUPERNOVAE SO ASTROPHYSICAL JOURNAL LA English DT Article DE hydrodynamics; nuclear reactions, nucleosynthesis, abundances; supernovae: general; white dwarfs ID ADAPTIVE MESH REFINEMENT; WHITE-DWARF MERGERS; DELAYED-DETONATION; DEFLAGRATION PHASE; SIMULATIONS; EVOLUTION; IGNITION; EXPLOSION; CODE; PROPAGATION AB We describe the detonation mechanism composing the "pulsationally assisted" gravitationally confined detonation (GCD) model of Type Ia supernovae. This model is analogous to the previous GCD model reported in Jordan et al.; however, the chosen initial conditions produce a substantively different detonation mechanism, resulting from a larger energy release during the deflagration phase. The resulting final kinetic energy and Ni-56 yields conform better to observational values than is the case for the "classical" GCD models. In the present class of models, the ignition of a deflagration phase leads to a rising, burning plume of ash. The ash breaks out of the surface of the white dwarf, flows laterally around the star, and converges on the collision region at the antipodal point from where it broke out. The amount of energy released during the deflagration phase is enough to cause the star to rapidly expand, so that when the ash reaches the antipodal point, the surface density is too low to initiate a detonation. Instead, as the ash flows into the collision region (while mixing with surface fuel), the star reaches its maximally expanded state and then contracts. The stellar contraction acts to increase the density of the star, including the density in the collision region. This both raises the temperature and density of the fuel-ash mixture in the collision region and ultimately leads to thermodynamic conditions that are necessary for the Zel'dovich gradient mechanism to produce a detonation. We demonstrate feasibility of this scenario with three three-dimensional (3D), full star simulations of this model using the FLASH code. We characterized the simulations by the energy released during the deflagration phase, which ranged from 38% to 78% of the white dwarf's binding energy. We show that the necessary conditions for detonation are achieved in all three of the models. C1 [Jordan, G. C.; Graziani, C.; Weide, K.; Norris, J.; Hudson, R.; Lamb, D. Q.] Univ Chicago, Flash Ctr Computat Sci, Chicago, IL 60637 USA. [Jordan, G. C.; Graziani, C.; Weide, K.; Lamb, D. Q.] Univ Chicago, Dept Astron & Astrophys, Chicago, IL 60637 USA. [Fisher, R. T.] Univ Massachusetts Dartmouth, Dept Phys, N Dartmouth, MA 02740 USA. [Townsley, D. M.] Univ Alabama, Dept Phys & Astron, Tuscaloosa, AL 35487 USA. [Meakin, C.] Univ Arizona, Steward Observ, Tucson, AZ 85721 USA. [Meakin, C.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Reid, L. B.] NTEC Environm Technol, Subiaco, WA 6008, Australia. [Lamb, D. Q.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. RP Jordan, GC (reprint author), Univ Chicago, Flash Ctr Computat Sci, Chicago, IL 60637 USA. RI Fisher, Robert/J-8667-2014; OI Fisher, Robert/0000-0001-8077-7255; Weide, Klaus/0000-0001-9869-9750 FU US Department of Energy (DOE) [B523820]; National Science Foundation [AST-0909132]; INCITE program at ALCF at ANL; Office of Science of the US Department of Energy [DE-AC02-06CH11357] FX The authors thank the FLASH Code Group, especially Chris Daley and Anshu Dubey for help with the development of and troubleshooting the code. We thank Brad Gallagher for creating Figures 1 and 2. We also thank Katherine Riley, Mike Papka, and the staff at the Argonne Leadership Computing Facility at Argonne National Laboratory for help running our large-scale simulations on Intrepid at ANL. This work was supported in part at the University of Chicago by the US Department of Energy (DOE) under Contract B523820 to the ASC Alliances Center for Astrophysical Nuclear Flashes, and in part by the National Science Foundation under Grant No. AST-0909132 for the "Petascale Computing of Thermonuclear Supernova Explosions." This research used computational resources awarded under the INCITE program at ALCF at ANL, which is supported by the Office of Science of the US Department of Energy under Contract No. DE-AC02-06CH11357. NR 66 TC 24 Z9 24 U1 0 U2 6 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X J9 ASTROPHYS J JI Astrophys. J. PD NOV 1 PY 2012 VL 759 IS 1 AR 53 DI 10.1088/0004-637X/759/1/53 PG 15 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 030JL UT WOS:000310566900053 ER PT J AU Roth, N Kasen, D Hopkins, PF Quataert, E AF Roth, Nathaniel Kasen, Daniel Hopkins, Philip F. Quataert, Eliot TI THREE-DIMENSIONAL RADIATIVE TRANSFER CALCULATIONS OF RADIATION FEEDBACK FROM MASSIVE BLACK HOLES: OUTFLOW OF MASS FROM THE DUSTY "TORUS" SO ASTROPHYSICAL JOURNAL LA English DT Article DE black hole physics; galaxies: active; galaxies: kinematics and dynamics; galaxies: nuclei; quasars: general; radiative transfer ID ACTIVE GALACTIC NUCLEI; ABSORBING COLUMN DENSITIES; XMM-NEWTON OBSERVATIONS; NARROW-LINE REGION; SEYFERT-GALAXIES; NGC 1068; VELOCITY DISPERSION; SCALE OUTFLOWS; OBSCURING TORI; HOST GALAXIES AB Observational and theoretical arguments suggest that the momentum carried in mass outflows from active galactic nuclei (AGNs) can reach several times L/c, corresponding to outflow rates of hundreds of solar masses per year. Radiation pressure on resonant absorption lines alone may not be sufficient to provide this momentum deposition, and the transfer of reprocessed IR radiation in dusty nuclear gas has been postulated to provide the extra enhancement. The efficacy of this mechanism, however, will be sensitive to multi-dimensional effects such as the tendency for the reprocessed radiation to preferentially escape along sightlines of lower column density. We use Monte Carlo radiative transfer calculations to determine the radiation force on dusty gas residing within approximately 30 parsecs from an accreting supermassive black hole. We calculate the net rate of momentum deposition in the surrounding gas and estimate the mass-loss rate in the resulting outflow as a function of solid angle for different black hole luminosities, sightline-averaged column densities, clumping parameters, and opening angles of the dusty gas. We find that these dust-driven winds carry momentum fluxes of 1-5 times L/c and correspond to mass-loss rates of 10-100 M-circle dot per year for a 10(8) M-circle dot black hole radiating at or near its Eddington limit. These results help to explain the origin of high velocity molecular and atomic outflows in local ultraluminous infrared galaxies and can inform numerical simulations of galaxy evolution including AGN feedback. C1 [Roth, Nathaniel; Kasen, Daniel; Quataert, Eliot] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Kasen, Daniel; Hopkins, Philip F.; Quataert, Eliot] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. [Kasen, Daniel; Hopkins, Philip F.; Quataert, Eliot] Univ Calif Berkeley, Theoret Astrophys Ctr, Berkeley, CA 94720 USA. [Kasen, Daniel] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. RP Roth, N (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM nathaniel.roth@berkeley.edu OI Roth, Nathaniel/0000-0002-6485-2259 FU Department of Energy Office of Science Graduate Fellowship Program (DOE SCGF); ORISE-ORAU [DE-AC05-06OR23100]; Department of Energy Office of Nuclear Physics Early Career Award; David and Lucile Packard Foundation; NASA [PF1-120083]; Office of Energy Research, Office of High Energy and Nuclear Physics, and Divisions of Nuclear Physics, of the U.S. Department of Energy [DE-AC02-05CH11231]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX We thank Jason Dexter, Claude-Andre Faucher-Giguere, and Nahum Arav for helpful conversations, along with the referee for thoughtful recommendations. N.R. is supported by the Department of Energy Office of Science Graduate Fellowship Program (DOE SCGF), made possible in part by the American Recovery and Reinvestment Act of 2009, administered by ORISE-ORAU under contract no. DE-AC05-06OR23100. D. K. was supported in part by a Department of Energy Office of Nuclear Physics Early Career Award. E. Q. was supported in part by the David and Lucile Packard Foundation. Support for P. F. H. was provided by NASA through Einstein Postdoctoral Fellowship Award Number PF1-120083 issued by the Chandra Xray Observatory Center, which is operated by the Smithsonian Astrophysical Observatory for and on behalf of NASA under contract NAS8-03060. This work is supported by the Director, Office of Energy Research, Office of High Energy and Nuclear Physics, and Divisions of Nuclear Physics, of the U.S. Department of Energy under contract No. DE-AC02-05CH11231. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under contract No. DE-AC02-05CH11231. NR 68 TC 23 Z9 23 U1 0 U2 8 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X J9 ASTROPHYS J JI Astrophys. J. PD NOV 1 PY 2012 VL 759 IS 1 AR 36 DI 10.1088/0004-637X/759/1/36 PG 15 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 030JL UT WOS:000310566900036 ER PT J AU Vallinotto, A AF Vallinotto, Alberto TI USING COSMIC MICROWAVE BACKGROUND LENSING TO CONSTRAIN THE MULTIPLICATIVE BIAS OF COSMIC SHEAR SO ASTROPHYSICAL JOURNAL LA English DT Article DE cosmic background radiation; cosmological parameters; cosmology: observations; large-scale structure of universe ID WEAK; POLARIZATION; PROSPECTS AB Weak gravitational lensing is one of the key probes of cosmology. Cosmic shear surveys aimed at measuring the distribution of matter in the universe are currently being carried out (Pan-STARRS) or planned for the coming decade (DES, LSST, EUCLID, WFIRST). Crucial to the success of these surveys is the control of systematics. In this work, a new method to constrain one such family of systematics, known as multiplicative bias, is proposed. This method exploits the cross-correlation between weak-lensing measurements from galaxy surveys and the ones obtained from high-resolution cosmic microwave background experiments. This cross-correlation is shown to have the power to break the degeneracy between the normalization of the matter power spectrum and the multiplicative bias of cosmic shear and to be able to constrain the latter to a few percent. C1 Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Vallinotto, A (reprint author), Los Alamos Natl Lab, T-2,MS B285, Los Alamos, NM 87545 USA. EM avalli@lanl.gov FU DOE at LANL [DE-AC52-06NA25396] FX A.V. is supported by DOE at LANL under contract DE-AC52-06NA25396. It is a pleasure to thank Salman Habib, Katrin Heitmann, Scott Dodelson, and Sudeep Das for a number of discussions throughout the development of this project. NR 21 TC 16 Z9 16 U1 0 U2 4 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X J9 ASTROPHYS J JI Astrophys. J. PD NOV 1 PY 2012 VL 759 IS 1 AR 32 DI 10.1088/0004-637X/759/1/32 PG 4 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 030JL UT WOS:000310566900032 ER PT J AU Xu, H Govoni, F Murgia, M Li, H Collins, DC Norman, ML Cen, RY Feretti, L Giovannini, G AF Xu, Hao Govoni, Federica Murgia, Matteo Li, Hui Collins, David C. Norman, Michael L. Cen, Renyue Feretti, Luigina Giovannini, Gabriele TI COMPARISONS OF COSMOLOGICAL MAGNETOHYDRODYNAMIC GALAXY CLUSTER SIMULATIONS TO RADIO OBSERVATIONS SO ASTROPHYSICAL JOURNAL LA English DT Article DE galaxies: clusters: general; large-scale structure of universe; magnetic fields; methods: numerical ID FIELD POWER SPECTRUM; ADAPTIVE MESH REFINEMENT; ACTIVE GALACTIC NUCLEI; HIGH-REDSHIFT QUASARS; MAGNETIC-FIELDS; X-RAY; FARADAY-ROTATION; STATISTICAL PROPERTIES; BLACK-HOLES; COOL CORES AB Radio observations of galaxy clusters show that there are mu G magnetic fields permeating the intracluster medium (ICM), but it is hard to accurately constrain the strength and structure of the magnetic fields without the help of advanced computer simulations. We present qualitative comparisons of synthetic Very Large Array observations of simulated galaxy clusters to radio observations of Faraday rotation measure (RM) and radio halos. The cluster formation is modeled using adaptive mesh refinement magnetohydrodynamic simulations with the assumption that the initial magnetic fields are injected into the ICM by active galactic nuclei (AGNs) at high redshift. In addition to simulated clusters in Xu et al., we present a new simulation with magnetic field injections from multiple AGNs. We find that the cluster with multiple injection sources is magnetized to a similar level as in previous simulations with a single AGN. The RM profiles from simulated clusters, both vertical bar RM vertical bar and the dispersion of RM (sigma(RM)), are consistent at a first order with the radial distribution from observations. The correlations between the sigma(RM) and X-ray surface brightness from simulations are in a broad agreement with the observations, although there is an indication that the simulated clusters could be slightly overdense and less magnetized with respect to those in the observed sample. In addition, the simulated radio halos agree with the observed correlations between the radio power versus the cluster X-ray luminosity and between the radio power versus the radio halo size. These studies show that the cluster-wide magnetic fields that originate from AGNs and are then amplified by the ICM turbulence match observations of magnetic fields in galaxy clusters. C1 [Xu, Hao; Li, Hui; Collins, David C.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Xu, Hao; Norman, Michael L.] Univ Calif San Diego, Ctr Astrophys & Space Sci, La Jolla, CA 92093 USA. [Govoni, Federica; Murgia, Matteo] INAF Osservatorio Astron Cagliari, I-09012 Capoterra, CA, Italy. [Cen, Renyue] Princeton Univ, Dept Astrophys Sci, Princeton, NJ 08544 USA. [Feretti, Luigina; Giovannini, Gabriele] INAF Ist Radioastron, I-40129 Bologna, Italy. [Giovannini, Gabriele] Univ Bologna, Dipartimento Astron, I-40127 Bologna, Italy. RP Xu, H (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM hao_xu@lanl.gov; fgovoni@oa-cagliari.inaf.it; matteo@oa-cagliari.inaf.it; hli@lanl.gov; dccollins@lanl.gov; mlnorman@ucsd.edu; cen@astro.princeton.edu; lferetti@ira.inaf.it; ggiovann@ira.inaf.it RI Xu, Hao/B-8734-2014; OI Xu, Hao/0000-0003-4084-9925; Govoni, Federica/0000-0003-3644-3084; Murgia, Matteo/0000-0002-4800-0806; Feretti, Luigina/0000-0003-0312-6285; Giovannini, Gabriele/0000-0003-4916-6362 FU LANL; DOE/Office of Fusion Energy Science through CMSO; Advanced Simulation and Computing Program (ASC); U.S. DOE [DE-AC52- 06NA25396]; NSF [AST-0708960, AST-0808184]; NASA [NNX11AI23G] FX H.X. and H. L. are supported by the LDRD and IGPP programs at LANL and by DOE/Office of Fusion Energy Science through CMSO. D. C. is supported by Advanced Simulation and Computing Program (ASC) and LANL which is operated by LANS, LLC for the NNSA of the U.S. DOE under Contract No. DE-AC52- 06NA25396. Computing resources were supplied by the National Science Foundation by an allocation TG-MCA04N012 on Kraken at the National Institute of Computational Sciences. ENZO+MHD is developed at the Laboratory for Computational Astrophysics, UCSD, with partial support from NSF grants AST-0708960 and AST-0808184 to M.L.N. F. G. and M. M. thank the LANL for the support and hospitality during the preparation of this work. R. C. is supported in part by NASA grant NNX11AI23G. NR 69 TC 9 Z9 9 U1 0 U2 7 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD NOV 1 PY 2012 VL 759 IS 1 AR 40 DI 10.1088/0004-637X/759/1/40 PG 16 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 030JL UT WOS:000310566900040 ER PT J AU Friesen, B Baron, E Branch, D Chen, B Parrent, JT Thomas, RC AF Friesen, Brian Baron, E. Branch, David Chen, Bin Parrent, Jerod T. Thomas, R. C. TI SUPERNOVA RESONANCE-SCATTERING LINE PROFILES IN THE ABSENCE OF A PHOTOSPHERE SO ASTROPHYSICAL JOURNAL SUPPLEMENT SERIES LA English DT Article DE line: formation; line: profiles; radiative transfer; supernovae: general ID RADIATIVE-TRANSFER CALCULATIONS; IA SUPERNOVAE; LIGHT CURVES; ASYMMETRIC EXPLOSION; SPECTRAL EVOLUTION; ELECTRON-CAPTURE; NEBULAR SPECTRA; SN 1987A; TIME; EJECTA AB In supernova (SN) spectroscopy relatively little attention has been given to the properties of optically thick spectral lines in epochs following the photosphere's recession. Most treatments and analyses of post-photospheric optical spectra of SNe assume that forbidden-line emission comprises most if not all spectral features. However, evidence exists that suggests that some spectra exhibit line profiles formed via optically thick resonance-scattering even months or years after the SN explosion. To explore this possibility, we present a geometrical approach to SN spectrum formation based on the "Elementary Supernova" model, wherein we investigate the characteristics of resonance-scattering in optically thick lines while replacing the photosphere with a transparent central core emitting non-blackbody continuum radiation, akin to the optical continuum provided by decaying Co-56 formed during the explosion. We develop the mathematical framework necessary for solving the radiative transfer equation under these conditions and calculate spectra for both isolated and blended lines. Our comparisons with analogous results from the Elementary Supernova code SYNOW reveal several marked differences in line formation. Most notably, resonance lines in these conditions form P Cygni-like profiles, but the emission peaks and absorption troughs shift redward and blueward, respectively, from the line's rest wavelength by a significant amount, despite the spherically symmetric distribution of the line optical depth in the ejecta. These properties and others that we find in this work could lead to misidentification of lines or misattribution of properties of line-forming material at post-photospheric times in SN optical spectra. C1 [Friesen, Brian; Baron, E.; Branch, David; Chen, Bin] Univ Oklahoma, Homer L Dodge Dept Phys Astron, Norman, OK 73019 USA. [Baron, E.] Hamburger Sternwarte, D-21029 Hamburg, Germany. [Baron, E.; Thomas, R. C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Cosmol Ctr, Computat Res Div, Berkeley, CA 94720 USA. [Baron, E.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Parrent, Jerod T.] Dartmouth Coll, Dept Phys & Astron, Wilder Lab 6127, Hanover, NH 03755 USA. [Parrent, Jerod T.] Las Cumbres Observ Global Telescope Network, Goleta, CA 93117 USA. RP Friesen, B (reprint author), Univ Oklahoma, Homer L Dodge Dept Phys Astron, 440 Brooks St,Rm 100, Norman, OK 73019 USA. OI Baron, Edward/0000-0001-5393-1608 FU NSF [AST-0707704]; US DOE [DE-FG02-07ER41517]; DFG [SFB 676, GRK 1354]; NASA from Space Telescope Science Institute [HST-GO-12298.05-A]; NASA [NAS5-26555] FX The referee's careful eye vastly improved the content of this work, for which we are grateful. This work was supported in part by NSF grant AST-0707704, and US DOE Grant DE-FG02-07ER41517, and by SFB 676, GRK 1354 from the DFG. Support for Program No. HST-GO-12298.05-A was provided by NASA through a grant from the Space Telescope Science Institute, which is operated by the Association of Universities for Research in Astronomy, Incorporated, under NASA contract NAS5-26555. This research has made use of NASA's Astrophysics Data System. NR 48 TC 5 Z9 5 U1 1 U2 3 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0067-0049 J9 ASTROPHYS J SUPPL S JI Astrophys. J. Suppl. Ser. PD NOV PY 2012 VL 203 IS 1 AR 12 DI 10.1088/0067-0049/203/1/12 PG 15 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 034YH UT WOS:000310908300012 ER PT J AU McComas, DJ Dayeh, MA Allegrini, F Bzowski, M DeMajistre, R Fujiki, K Funsten, HO Fuselier, SA Gruntman, M Janzen, PH Kubiak, MA Kucharek, H Livadiotis, G Mobius, E Reisenfeld, DB Reno, M Schwadron, NA Sokol, JM Tokumaru, M AF McComas, D. J. Dayeh, M. A. Allegrini, F. Bzowski, M. DeMajistre, R. Fujiki, K. Funsten, H. O. Fuselier, S. A. Gruntman, M. Janzen, P. H. Kubiak, M. A. Kucharek, H. Livadiotis, G. Moebius, E. Reisenfeld, D. B. Reno, M. Schwadron, N. A. Sokol, J. M. Tokumaru, M. TI THE FIRST THREE YEARS OF IBEX OBSERVATIONS AND OUR EVOLVING HELIOSPHERE SO ASTROPHYSICAL JOURNAL SUPPLEMENT SERIES LA English DT Article DE ISM: general; ISM: magnetic fields; plasmas; solar wind; Sun: heliosphere; stars: atmospheres ID INTERSTELLAR-BOUNDARY-EXPLORER; NEUTRAL ATOM SPECTRA; SLOW SOLAR-WIND; PICK-UP IONS; OUTER HELIOSHEATH; 1 AU; LO OBSERVATIONS; RIBBON; HYDROGEN; FLUX AB This study provides, for the first time, complete and validated observations from the first three years (2009-2011) of the Interstellar Boundary Explorer (IBEX) mission. Energetic neutral atom (ENA) fluxes are corrected for both the time-variable cosmic ray background and for orbit-by-orbit variations in their probability of surviving en route from the outer heliosphere in to 1 AU where IBEX observes them. In addition to showing all six six-month maps, we introduce new annual ram and anti-ram maps, which can be produced without the need for algorithm-dependent Compton-Getting corrections. Together, the ENA maps, data, and supporting documentation presented here support the full release of these data to the broader scientific community and provide the citable reference for them. In addition, we show that heliospheric ENA emissions have been decreasing over the epoch from 2009 to 2011 with the IBEX Ribbon decreasing by the largest fraction and only the heliotail (which is offset from the down wind direction by the interstellar magnetic field) showing essentially no reduction and actually some increase. Finally, we show how the much more complete observations provided here strongly indicate a quite direct and latitude-dependent solar wind source of the Ribbon. C1 [McComas, D. J.; Dayeh, M. A.; Allegrini, F.; Fuselier, S. A.; Livadiotis, G.; Reno, M.; Schwadron, N. A.] SW Res Inst, San Antonio, TX 78228 USA. [McComas, D. J.; Allegrini, F.] Univ Texas San Antonio, Dept Phys & Astron, San Antonio, TX 78249 USA. [Bzowski, M.; Kubiak, M. A.; Sokol, J. M.] Polish Acad Sci, Space Res Ctr, PL-00716 Warsaw, Poland. [DeMajistre, R.] Johns Hopkins Univ, Appl Phys Lab, Laurel, MD 20723 USA. [Fujiki, K.; Tokumaru, M.] Nagoya Univ, Solar Terr Environm Lab, Nagoya, Aichi 4648601, Japan. [Funsten, H. O.] Los Alamos Natl Lab, Intelligence & Space Res Div, Los Alamos, NM 87545 USA. [Gruntman, M.] Univ So Calif, Viterbi Sch Engn, Dept Astronaut Engn, Los Angeles, CA 90089 USA. [Janzen, P. H.; Reisenfeld, D. B.] Univ Montana, Dept Phys & Astron, Missoula, MT 59812 USA. [Kucharek, H.; Moebius, E.; Schwadron, N. A.] Univ New Hampshire, Ctr Space Sci, Durham, NH 03824 USA. [Reno, M.] Austin Mission Consulting, Austin, TX 78749 USA. RP McComas, DJ (reprint author), SW Res Inst, PO Drawer 28510, San Antonio, TX 78228 USA. EM dmccomas@swri.org RI Funsten, Herbert/A-5702-2015; Reisenfeld, Daniel/F-7614-2015; Gruntman, Mike/A-5426-2008; Sokol, Justyna/K-2892-2015; OI Funsten, Herbert/0000-0002-6817-1039; Gruntman, Mike/0000-0002-0830-010X; Moebius, Eberhard/0000-0002-2745-6978 FU NASA's Explorer Program; Polish Ministry for Science and Higher Education Grant [NS-1260-11-09]; United States National Science Foundation [ANT-0739620, ANT-0838839]; University of Delaware Department of Physics and Astronomy; Bartol Research Institute; U.S. Department of Energy through LANL's Laboratory Directed Research and Development (LDRD) Program; Institute Geophysics and Planetary Physics FX We thank all of the outstanding men and women who have made the IBEX mission such a wonderful success. This work was carried out as a part of the IBEX project, with support from NASA's Explorer Program and Polish Ministry for Science and Higher Education Grant NS-1260-11-09. We also gratefully acknowledge the McMurdo data from the Bartol Research Institute neutron monitor program, which is supported by the United States National Science Foundation under grants ANT-0739620 and ANT-0838839, and by the University of Delaware Department of Physics and Astronomy and Bartol Research Institute. E. Mobius gratefully acknowledges the support of the U.S. Department of Energy through LANL's Laboratory Directed Research and Development (LDRD) Program and Institute Geophysics and Planetary Physics. NR 68 TC 68 Z9 69 U1 0 U2 16 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0067-0049 EI 1538-4365 J9 ASTROPHYS J SUPPL S JI Astrophys. J. Suppl. Ser. PD NOV PY 2012 VL 203 IS 1 AR 1 DI 10.1088/0067-0049/203/1/1 PG 36 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 034YH UT WOS:000310908300001 ER PT J AU Bu, Q Lei, HW Zacher, AH Wang, L Ren, SJ Liang, J Wei, Y Liu, YP Tang, J Zhang, Q Ruan, R AF Bu, Quan Lei, Hanwu Zacher, Alan H. Wang, Lu Ren, Shoujie Liang, Jing Wei, Yi Liu, Yupeng Tang, Juming Zhang, Qin Ruan, Roger TI A review of catalytic hydrodeoxygenation of lignin-derived phenols from biomass pyrolysis SO BIORESOURCE TECHNOLOGY LA English DT Review DE Lignin-derived phenols; Catalytic hydrodeoxygenation (HDO); Pyrolysis; Mechanism; Kinetics ID METHYL-SUBSTITUTED PHENOLS; BIO-OIL; TRANSPORTATION FUELS; MODEL COMPOUNDS; CHEMICALS; HYDROGEN; DEACTIVATION; CONVERSION; FRACTIONS; KINETICS AB Catalytic hydrodeoxygenation (HDO) of lignin-derived phenols which are the lowest reactive chemical compounds in biomass pyrolysis oils has been reviewed. The hydrodeoxygenation (HDO) catalysts have been discussed including traditional HDO catalysts such as CoMo/Al2O3 and NiMo/Al2O3 catalysts and transition metal catalysts (noble metals). The mechanism of HDO of lignin-derived phenols was analyzed on the basis of different model compounds. The kinetics of HDO of different lignin-derived model compounds has been investigated. The diversity of bio-oils leads to the complexities of HDO kinetics. The techno-economic analysis indicates that a series of major technical and economical efforts still have to be investigated in details before scaling up the HDO of lignin-derived phenols in existed refinery infrastructure. Examples of future investigation of HDO include significant challenges of improving catalysts and optimum operation conditions, further understanding of kinetics of complex bio-oils, and the availability of sustainable and cost-effective hydrogen source. (C) 2012 Elsevier Ltd. All rights reserved. C1 [Bu, Quan; Lei, Hanwu; Wang, Lu; Ren, Shoujie; Liang, Jing; Wei, Yi; Liu, Yupeng; Tang, Juming; Zhang, Qin] Washington State Univ, Dept Biol Syst Engn, Bioprod Sci & Engn Lab, Richland, WA 99354 USA. [Zacher, Alan H.] Pacific NW Natl Lab, Richland, WA 99354 USA. [Ruan, Roger] Univ Minnesota, Dept Bioprod & Biosyst Engn, St Paul, MN 55108 USA. RP Lei, HW (reprint author), Washington State Univ, Dept Biol Syst Engn, Bioprod Sci & Engn Lab, Richland, WA 99354 USA. EM hlei@tricity.wsu.edu RI ren, shoujie/P-1384-2014; OI Ruan, Roger/0000-0001-8835-2649 FU Office of Research and Department of Biological Systems Engineering at Washington State University FX This work was supported in partial by the Office of Research and Department of Biological Systems Engineering at Washington State University. NR 74 TC 123 Z9 128 U1 29 U2 389 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0960-8524 EI 1873-2976 J9 BIORESOURCE TECHNOL JI Bioresour. Technol. PD NOV PY 2012 VL 124 BP 470 EP 477 DI 10.1016/j.biortech.2012.08.089 PG 8 WC Agricultural Engineering; Biotechnology & Applied Microbiology; Energy & Fuels SC Agriculture; Biotechnology & Applied Microbiology; Energy & Fuels GA 038LA UT WOS:000311175000061 PM 23021958 ER PT J AU Chen, XN Zhang, YS Wang, YL Zhou, W Knight, DA Yisgedu, TB Huang, ZG Lingam, HK Billet, B Udovic, TJ Brown, GM Shore, SG Wolverton, C Zhao, JC AF Chen, Xuenian Zhang, Yongsheng Wang, Yongli Zhou, Wei Knight, Douglas A. Yisgedu, Teshome B. Huang, Zhenguo Lingam, Hima K. Billet, Beau Udovic, Terrence J. Brown, Gilbert M. Shore, Sheldon G. Wolverton, Christopher Zhao, Ji-Cheng TI Structure determination of an amorphous compound AlB4H11 SO CHEMICAL SCIENCE LA English DT Article ID THERMAL-DECOMPOSITION; ALUMINIUM BOROHYDRIDE; MOLECULAR-STRUCTURE; DIBORANE PYROLYSIS; AMMONIA TRIBORANE; HYDROGEN STORAGE; BORANES; INTERCONVERSION; COMPLEXES; LIGANDS AB The structure of the amorphous aluminoborane compound AlB4H11 was identified through a collaborative study closely coupling a first-principles density functional based approach with experimental measurements using IR, NMR, and neutron vibrational spectroscopy (NVS). The AlB4H11 structure was found to contain distinct [BH4] and [B3H7] units without any [AlH4] units. It forms a -[B3H7]-Al(BH4)- polymer chain with the [BH4] units twisted relative to each other perpendicular to the chain direction and bonded to Al, and a chain backbone consists of [B3H7] and Al where the [B3H7] unit exhibits a triangular boron configuration. The computed lowest energy structure shows good agreement with results of IR, NVS and NMR spectra; this agreement demonstrates the extended applicability of the structure prediction approach to the prediction of even amorphous compounds. C1 [Zhou, Wei; Udovic, Terrence J.] Natl Inst Stand & Technol, NIST Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Chen, Xuenian; Yisgedu, Teshome B.; Huang, Zhenguo; Lingam, Hima K.; Billet, Beau; Zhao, Ji-Cheng] Ohio State Univ, Dept Mat Sci & Engn, Columbus, OH 43210 USA. [Chen, Xuenian; Shore, Sheldon G.] Ohio State Univ, Dept Chem, Columbus, OH 43210 USA. [Zhang, Yongsheng; Wang, Yongli; Wolverton, Christopher] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. [Zhou, Wei] Univ Maryland, Dept Mat Sci & Engn, College Pk, MD 20742 USA. [Knight, Douglas A.] Savannah River Natl Lab, Aiken, SC 29808 USA. [Brown, Gilbert M.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Udovic, TJ (reprint author), Natl Inst Stand & Technol, NIST Ctr Neutron Res, Gaithersburg, MD 20899 USA. EM terrence.udovic@nist.gov; browngm1@ornl.gov; shore.1@osu.edu; c-wolverton@northwestern.edu; zhao.199@osu.edu RI Zhou, Wei/C-6504-2008; Zhao, Ji-Cheng (JC)/H-4387-2012; Wolverton, Christopher/B-7542-2009; Huang, Zhenguo/F-4483-2016; OI Zhou, Wei/0000-0002-5461-3617; Zhao, Ji-Cheng (JC)/0000-0002-4426-1080; Knight, David/0000-0001-5510-6265 FU U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy [DE-FC3605GO15062]; U.S. Department of Energy [DE-FC36-08GO18136, DE-FG02-07ER46433, DE-EE0002978, DE-AI-01-05EE11104]; Ford Motor Company; DOE by UT Battelle, LLC [DE-AC05-00OR22725]; Office of Energy Efficiency and Renewable Energy, Office of Hydrogen, Fuel Cell, and Infrastructure Technologies of DOE; DOE Metal Hydride Center of Excellence FX This work was supported by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, under Contract no. DE-FC3605GO15062. Y. Z., Y. W. and C. W. gratefully acknowledge financial support from the U.S. Department of Energy under grant nos DE-FC36-08GO18136 and DE-FG02-07ER46433, and funding from Ford Motor Company under the University Research Program. T.J.U. and W.Z. gratefully acknowledge financial support from the U.S. Department of Energy under grant nos DE-EE0002978 and DE-AI-01-05EE11104. ORNL is managed and operated for the DOE by UT Battelle, LLC under contract DE-AC05-00OR22725. Research at ORNL is also supported by the Office of Energy Efficiency and Renewable Energy, Office of Hydrogen, Fuel Cell, and Infrastructure Technologies of DOE in conjunction with the DOE Metal Hydride Center of Excellence. The participation of Douglas A. Knight was made possible by appointment in the ORNL Postgraduate Program administrated by the Oak Ridge Institute for Science and Education. The authors from OSU are grateful to Profs. Edward A. Meyers and Thomas Evans for their very valuable comments. Critical comments of Dr Robert C. Bowman, Jr are also greatly acknowledged. NR 68 TC 13 Z9 13 U1 1 U2 42 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2041-6520 J9 CHEM SCI JI Chem. Sci. PD NOV PY 2012 VL 3 IS 11 BP 3183 EP 3191 DI 10.1039/c2sc21100a PG 9 WC Chemistry, Multidisciplinary SC Chemistry GA 036YL UT WOS:000311068100008 ER PT J AU Zhao, D Shui, JL Chen, C Chen, XQ Reprogle, BM Wang, DP Liu, DJ AF Zhao, Dan Shui, Jiang-Lan Chen, Chen Chen, Xinqi Reprogle, Briana M. Wang, Dapeng Liu, Di-Jia TI Iron imidazolate framework as precursor for electrocatalysts in polymer electrolyte membrane fuel cells SO CHEMICAL SCIENCE LA English DT Article ID OXYGEN REDUCTION CATALYSTS; FE-BASED CATALYSTS; X-RAY-DIFFRACTION; METAL-ORGANIC FRAMEWORKS; CATHODE CATALYST; RAMAN-SPECTROSCOPY; PEMFC SCIENCE; QUANTUM JUMPS; CARBON; PYROLYSIS AB The extensive use of Pt and platinum group metals (PGM) as electrocatalysts poses a significant cost barrier for the commercialization of polymer electrolyte membrane fuel cells (PEMFC). Replacing Pt with non-PGM electrocatalysts is a long-term pursuit of the scientific community. In this study, non-PGM cathode electrocatalysts for PEMFC were prepared by pyrolyzing an iron imidazolate framework. The new catalyst demonstrated excellent activity towards oxygen reduction reaction in the acidic medium. The catalytic activity was further improved by mixing with a zinc imidazolate framework, ZIF-8. The membrane electrode assembly made of such catalyst as the cathode demonstrated an onset potential of 0.977 V and measured volumetric current density of 12 A cm(-3) at 0.8 V in a single cell test. C1 [Zhao, Dan; Shui, Jiang-Lan; Chen, Chen; Reprogle, Briana M.; Wang, Dapeng; Liu, Di-Jia] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Chen, Xinqi] Northwestern Univ, Dept Mech Engn, Evanston, IL 60208 USA. RP Liu, DJ (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM djliu@anl.gov RI Zhao, Dan/D-5975-2011 OI Zhao, Dan/0000-0002-4427-2150 FU UChicago Argonne, LLC [DE-AC02-06CH11357]; Argonne National Laboratory FX The authors wish to thank Dr Deborah J. Myers for her assistance in the single cell test and Dr Jun Lu for his advice on XPS data fitting. The electron microscopy was accomplished at the Electron Microscopy Center for Materials Research at Argonne National Laboratory, a U.S. Department of Energy Office of Science Laboratory operated under Contract no. DE-AC02-06CH11357 by UChicago Argonne, LLC. The financial support of Argonne National Laboratory is gratefully acknowledged. NR 47 TC 84 Z9 84 U1 24 U2 189 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 2041-6520 J9 CHEM SCI JI Chem. Sci. PD NOV PY 2012 VL 3 IS 11 BP 3200 EP 3205 DI 10.1039/c2sc20657a PG 6 WC Chemistry, Multidisciplinary SC Chemistry GA 036YL UT WOS:000311068100011 ER PT J AU Ostrowski, J Wang, JH AF Ostrowski, James Wang, Jianhui TI Network reduction in the Transmission-Constrained Unit Commitment problem SO COMPUTERS & INDUSTRIAL ENGINEERING LA English DT Article DE Unit Commitment; Transmission network; Mixed Integer Linear Programming; Network reduction ID BENDERS DECOMPOSITION AB This paper examines a preprocessing technique for a Mixed Integer Linear Programming (MILP) formulation of the Transmission-Constrained Unit Commitment problem (TC-UC). Incorporating transmission constraints into the Unit Commitment problem can significantly increase the size and difficulty of the problem. By examining the structure of the transmission network, variables that have no impact on the quality of the overall solution can be identified and removed. This preprocessing can reduce the time needed to solve the linear programming relaxation of the MILP, and as a result, the MILP itself. Illinois's transmission network was used to test the benefit of the proposed technique. Preprocessing was able to remove 30% of the buses in the transmission network. This reduction led to a significant decrease in the time needed to solve a 24 h TC-UC problem. An added benefit of the preprocessing is that symmetry can be introduced into the problem. Identifying this symmetry and exploiting it can improve overall solution times even further. (C) 2012 Published by Elsevier Ltd. C1 [Ostrowski, James] Univ Tennessee, Knoxville, TN 37996 USA. [Wang, Jianhui] Argonne Natl Lab, Argonne, IL 60439 USA. RP Ostrowski, J (reprint author), Univ Tennessee, 1425 S Stadium Dr,409 E Stadium Hall, Knoxville, TN 37996 USA. EM jostrows@utk.edu; jianhui.wang@anl.gov OI Ostrowski, James/0000-0001-5636-555X NR 18 TC 3 Z9 4 U1 0 U2 2 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-8352 J9 COMPUT IND ENG JI Comput. Ind. Eng. PD NOV PY 2012 VL 63 IS 3 SI SI BP 702 EP 707 DI 10.1016/j.cie.2012.02.013 PG 6 WC Computer Science, Interdisciplinary Applications; Engineering, Industrial SC Computer Science; Engineering GA 018AH UT WOS:000309631800018 ER PT J AU He, YY Wang, LZ Wang, JH AF He, Yanyi Wang, Lizhi Wang, Jianhui TI Cap-and-trade vs. carbon taxes: A quantitative comparison from a generation expansion planning perspective SO COMPUTERS & INDUSTRIAL ENGINEERING LA English DT Article DE Cap-and-trade; Carbon tax; Generation expansion planning ID POWER-SYSTEMS; CUT ALGORITHM; EMISSIONS; SCHEME; PRICES; MARKET AB We compare the effectiveness and efficiency of cap-and-trade and carbon tax policies in a generation expansion planning framework. The effectiveness refers to a policy's capability to control the amount of carbon emissions, and the efficiency is measured with respect to seven criteria: average emissions price, actual emissions, renewable energy portfolio, total generation, total profit of Gencos and grid owner, economic welfare, and emissions adjusted economic welfare. Cap-and-trade and four variations of carbon tax policies are integrated in a game-theoretic based generation expansion planning model to assess their impacts on new investment in renewable energy generation capacity. A case study is conducted on a 30-bus test system, and numerical results provide insights on the advantages and disadvantages of these policies. (C) 2011 Elsevier Ltd. All rights reserved. C1 [He, Yanyi; Wang, Lizhi] Iowa State Univ, Ames, IA 50011 USA. [Wang, Jianhui] Argonne Natl Lab, Argonne, IL 60439 USA. RP Wang, LZ (reprint author), Iowa State Univ, Ames, IA 50011 USA. EM lzwang@iastate.edu FU US National Science Foundation [EFRI-0835989]; Power Systems Engineering Research Center [M-28] FX This research is partially supported by the US National Science Foundation under Grant EFRI-0835989 and by the Power Systems Engineering Research Center under Grant M-28. NR 28 TC 19 Z9 21 U1 7 U2 58 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0360-8352 J9 COMPUT IND ENG JI Comput. Ind. Eng. PD NOV PY 2012 VL 63 IS 3 SI SI BP 708 EP 716 DI 10.1016/j.cie.2011.10.005 PG 9 WC Computer Science, Interdisciplinary Applications; Engineering, Industrial SC Computer Science; Engineering GA 018AH UT WOS:000309631800019 ER PT J AU Brown, JP Pender, J Wiser, R Lantz, E Hoen, B AF Brown, Jason P. Pender, John Wiser, Ryan Lantz, Eric Hoen, Ben TI Ex post analysis of economic impacts from wind power development in U.S. counties SO ENERGY ECONOMICS LA English DT Article DE Wind power; Economic development; Ex post analysis ID UNITED-STATES; RENEWABLE ENERGY; GROWTH; EMPLOYMENT; US; AMENITIES; GERMANY; MODELS AB Wind power development has surged in recent years in the United States. Policymakers and economic development practitioners to date have typically relied upon project-level case studies or modeled input-output estimates to assess the economic development impacts from wind power, often focusing on potential local, state-wide, or national employment or earnings impacts. Building on this literature, we conduct an ex post econometric analysis of the county-level economic development impacts of wind power installations from 2000 through 2008 in a large, wind-rich region in the country. Taking into account factors influencing wind turbine location, we find an aggregate increase in county-level personal income and employment of approximately 511,000 and 0.5 jobs per megawatt of wind power capacity installed over the sample period of 2000 to 2008. These estimates appear broadly consistent with modeled input-output results, and translate to a median increase in total county personal income and employment of 0.2% and 0.4% for counties with installed wind power over the same period. Published by Elsevier B.V. C1 [Brown, Jason P.; Pender, John] USDA, Econ Res Serv, Washington, DC 20024 USA. [Wiser, Ryan] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Lantz, Eric] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Hoen, Ben] Lawrence Berkeley Natl Lab, Milan, NY USA. RP Brown, JP (reprint author), USDA, Econ Res Serv, 355 E St SW, Washington, DC 20024 USA. EM jbrown@ers.usda.gov; jpender@ers.usda.gov; RHWiser@lbl.gov; eric.lantz@nrel.gov; BHoen@lbl.gov NR 55 TC 12 Z9 13 U1 7 U2 37 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0140-9883 J9 ENERG ECON JI Energy Econ. PD NOV PY 2012 VL 34 IS 6 BP 1743 EP 1754 DI 10.1016/j.eneco.2012.07.010 PG 12 WC Economics SC Business & Economics GA 035JX UT WOS:000310943800001 ER PT J AU Blum, H Legey, LFL AF Blum, Helcio Legey, Luiz F. L. TI The challenging economics of energy security: Ensuring energy benefits in support to sustainable development SO ENERGY ECONOMICS LA English DT Article DE Energy security; Energy policies; Sustainable development ID SOCIAL-ECOLOGICAL SYSTEMS; RESILIENCE; INDICATORS; DIVERSITY; COUNTRIES AB Energy is a key-resource to economic development and is required to be available continuously and in adequate amounts. Also, it is expected to be affordable and environmentally friendly. Ensuring this is a challenge, yet strategic to maintain economies running under a sustainable pattern. Energy security is neither a new concept, nor a new concern. However, because of new issues, it requires a novel, broader approach. Such an approach should address both demand (security of supply) and supply (security of demand) sides, as well as take into account energy scarcity situations and surplus opportunities. In addition, it should allow for both private (markets) and public (policies and regulations) initiatives. This paper presents a theoretical and practical basis for the economics of energy security. Energy security is defined, in this context, as the ability of an economy to provide sufficient, affordable and environmentally sustainable energy services so as to maintain a maximum welfare state, even when issues would press it otherwise. We introduce the notion of energy security gap to represent the economy's failure to show such ability. Additionally, we also propose a framework to support the evaluation, planning and implementation of energy security in an economy. This framework relies on the concepts of resilience, adaptability and transformability (Walker et al, 2004) to prescribe indicators to assess the energy security of an economy. Furthermore, it proposes mechanisms to enhance energy security, as well as a continuous process to increasingly achieve this. (C) 2012 Elsevier B.V. All rights reserved. C1 [Blum, Helcio; Legey, Luiz F. L.] Univ Fed Rio de Janeiro, Grad Sch Engn, Energy Planning Program, BR-21941 Rio De Janeiro, Brazil. [Blum, Helcio] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. RP Blum, H (reprint author), 1 Cyclotron Rd,Mail Stop 90R4C00, Berkeley, CA 94720 USA. EM hblum@lbl.gov NR 84 TC 21 Z9 22 U1 0 U2 39 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0140-9883 J9 ENERG ECON JI Energy Econ. PD NOV PY 2012 VL 34 IS 6 BP 1982 EP 1989 DI 10.1016/j.eneco.2012.08.013 PG 8 WC Economics SC Business & Economics GA 035JX UT WOS:000310943800026 ER PT J AU Tan, Y Maxwell, E Tan, YX Hu, H Benson, G Aizikov, K Conley, S Staples, G Slysz, G Smith, R Zaia, J AF Tan, Yan Maxwell, Evan Tan, Yuxiang Hu, Han Benson, Gary Aizikov, Konstantin Conley, Shannon Staples, Gregory Slysz, Gordon Smith, Richard Zaia, Joseph TI GlycReSoft: A software tool for processing glycomics and glycopeptidomics LC/MS profiling data SO GLYCOBIOLOGY LA English DT Meeting Abstract CT Joint Meeting of the Society-for-Glycobiology and American-Society-for-Matrix-Biology CY NOV 11-14, 2012 CL San Diego, CA SP Soc Glycobiol, Amer Soc Matrix Biol C1 [Tan, Yan; Maxwell, Evan; Tan, Yuxiang; Hu, Han; Benson, Gary; Aizikov, Konstantin; Conley, Shannon; Staples, Gregory; Zaia, Joseph] Boston Univ, Boston, MA 02215 USA. [Slysz, Gordon; Smith, Richard] Pacific NW Natl Lab, Richland, WA 99352 USA. NR 0 TC 0 Z9 0 U1 0 U2 4 PU OXFORD UNIV PRESS INC PI CARY PA JOURNALS DEPT, 2001 EVANS RD, CARY, NC 27513 USA SN 0959-6658 J9 GLYCOBIOLOGY JI Glycobiology PD NOV PY 2012 VL 22 IS 11 BP 1616 EP 1617 PG 2 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA 027QS UT WOS:000310368700295 ER PT J AU Farzbod, F Hurley, DH AF Farzbod, Farhad Hurley, David H. TI Using Eigenmodes to Perform the Inverse Problem Associated With Resonant Ultrasound Spectroscopy SO IEEE TRANSACTIONS ON ULTRASONICS FERROELECTRICS AND FREQUENCY CONTROL LA English DT Article ID ELASTIC-CONSTANTS; CRYSTALLOGRAPHIC ORIENTATION; OPTICAL-DETECTION; SINGLE-CRYSTALS; SOLIDS; MICROSCOPY; MODULI; MODES AB In principle, resonant ultrasonic spectroscopy (RUS) can be used to characterize any parameter that influences the mechanical resonant response of a sample. Examples include the elastic constants, sample dimensions, and crystal orientation. Extracting the parameter of interest involves performing the inverse problem, which typically entails an iterative routine that compares calculated and measured eigenfrequencies. Here, we propose an alternative method based on laser-based resonant ultrasound spectroscopy (LRUS) that uses the eigenmodes. LRUS uses a pulsed laser to thermoelastically excite ultrasound and an interferometer to detect out-of-plane displacement associated with ultrasonic resonances. By raster scanning the probe along the sample surface, an image of the out-of-plane displacement pattern (i.e., eigenmode) is obtained. As an example of this method, we describe a technique to calculate the crystallographic orientation of a single-crystal high-purity copper sample. The crystallographic orientation is computed by comparing theoretical and experimental eigenmodes. The computed angle is shown to be in very good agreement with the angle obtained using electron backscatter diffraction. In addition, a comparison is made using eigenfrequencies and eigenmodes to calculate the crystallographic orientation. It is found for this particular application, the eigenmode method has superior sensitivity to crystal orientation. C1 [Farzbod, Farhad; Hurley, David H.] Idaho Natl Lab, Dept Mat Sci & Engn, Idaho Falls, ID 83415 USA. RP Farzbod, F (reprint author), Idaho Natl Lab, Dept Mat Sci & Engn, Idaho Falls, ID 83415 USA. EM farzbod@ieee.org NR 31 TC 4 Z9 4 U1 1 U2 15 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0885-3010 J9 IEEE T ULTRASON FERR JI IEEE Trans. Ultrason. Ferroelectr. Freq. Control PD NOV PY 2012 VL 59 IS 11 BP 2470 EP 2475 DI 10.1109/TUFFC.2012.2479 PG 6 WC Acoustics; Engineering, Electrical & Electronic SC Acoustics; Engineering GA 035WC UT WOS:000310981600010 PM 23192810 ER PT J AU Zhou, DHH Nieuwkoop, AJ Berthold, DA Comellas, G Sperling, LJ Tang, M Shah, GJ Brea, EJ Lemkau, LR Rienstra, CM AF Zhou, Donghua H. Nieuwkoop, Andrew J. Berthold, Deborah A. Comellas, Gemma Sperling, Lindsay J. Tang, Ming Shah, Gautam J. Brea, Elliott J. Lemkau, Luisel R. Rienstra, Chad M. TI Solid-state NMR analysis of membrane proteins and protein aggregates by proton detected spectroscopy SO JOURNAL OF BIOMOLECULAR NMR LA English DT Article DE Chemical assignment; Solid-state NMR; Proton detection; Magic-angle spinning ID ANGLE-SPINNING NMR; ALPHA-SYNUCLEIN FIBRILS; TRIPLE-RESONANCE NMR; ISOTOPICALLY ENRICHED PROTEINS; SEQUENTIAL BACKBONE ASSIGNMENT; IMMUNOGLOBULIN BINDING DOMAIN; CHEMICAL-SHIFT ASSIGNMENTS; LARGER PROTEINS; SENSITIVITY ENHANCEMENT; PERDEUTERATED PROTEINS AB Solid-state NMR has emerged as an important tool for structural biology and chemistry, capable of solving atomic-resolution structures for proteins in membrane-bound and aggregated states. Proton detection methods have been recently realized under fast magic-angle spinning conditions, providing large sensitivity enhancements for efficient examination of uniformly labeled proteins. The first and often most challenging step of protein structure determination by NMR is the site-specific resonance assignment. Here we demonstrate resonance assignments based on high-sensitivity proton-detected three-dimensional experiments for samples of different physical states, including a fully-protonated small protein (GB1, 6 kDa), a deuterated microcrystalline protein (DsbA, 21 kDa), a membrane protein (DsbB, 20 kDa) prepared in a lipid environment, and the extended core of a fibrillar protein (alpha-synuclein, 14 kDa). In our implementation of these experiments, including CONH, CO(CA)NH, CANH, CA(CO)NH, CBCANH, and CBCA(CO)NH, dipolar-based polarization transfer methods have been chosen for optimal efficiency for relatively high protonation levels (full protonation or 100 % amide proton), fast magic-angle spinning conditions (40 kHz) and moderate proton decoupling power levels. Each H-N pair correlates exclusively to either intra- or inter-residue carbons, but not both, to maximize spectral resolution. Experiment time can be reduced by at least a factor of 10 by using proton detection in comparison to carbon detection. These high-sensitivity experiments are especially important for membrane proteins, which often have rather low expression yield. Proton-detection based experiments are expected to play an important role in accelerating protein structure elucidation by solid-state NMR with the improved sensitivity and resolution. C1 [Zhou, Donghua H.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74074 USA. [Nieuwkoop, Andrew J.; Berthold, Deborah A.; Sperling, Lindsay J.; Tang, Ming; Shah, Gautam J.; Brea, Elliott J.; Lemkau, Luisel R.; Rienstra, Chad M.] Univ Illinois, Dept Chem, Urbana, IL 61801 USA. [Nieuwkoop, Andrew J.] Leibniz Inst Mol Pharmacol, D-13125 Berlin, Germany. [Comellas, Gemma; Rienstra, Chad M.] Univ Illinois, Ctr Biophys & Computat Biol, Urbana, IL 61801 USA. [Sperling, Lindsay J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Zhou, DHH (reprint author), Oklahoma State Univ, Dept Phys, Stillwater, OK 74074 USA. EM donghua@okstate.edu; rienstra@illinois.edu RI Tang, Ming/A-5348-2010 OI Tang, Ming/0000-0001-7479-6206 FU National Institutes of Health [R01 GM-75937, R01 GM-73770, R15 GM-097713] FX We thank the National Institutes of Health for financial support (R01 GM-75937 and R01 GM-73770 to C. M. R and R15 GM-097713 to D.H.Z.). We also thank the NMR Facility at the School of Chemical Sciences, University of Illinois at Urbana-Champaign. NR 76 TC 51 Z9 51 U1 1 U2 48 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0925-2738 J9 J BIOMOL NMR JI J. Biomol. NMR PD NOV PY 2012 VL 54 IS 3 BP 291 EP 305 DI 10.1007/s10858-012-9672-z PG 15 WC Biochemistry & Molecular Biology; Spectroscopy SC Biochemistry & Molecular Biology; Spectroscopy GA 027WY UT WOS:000310386000007 PM 22986689 ER PT J AU Chae, KH Kravtsov, AV Frieman, JA Bernardi, M AF Chae, Kyu-Hyun Kravtsov, Andrey V. Frieman, Joshua A. Bernardi, Mariangela TI Semi-empirical catalog of early-type galaxy-halo systems: dark matter density profiles, halo contraction and dark matter annihilation strength SO JOURNAL OF COSMOLOGY AND ASTROPARTICLE PHYSICS LA English DT Article DE galaxy dynamics; galaxy formation; dark matter experiments ID INITIAL MASS FUNCTION; DIGITAL SKY SURVEY; ELLIPTIC GALAXIES; STELLAR MASS; LAMBDA-CDM; X-RAY; ADIABATIC CONTRACTION; SATELLITE KINEMATICS; LENTICULAR GALAXIES; FUNDAMENTAL PLANE AB With Sloan Digital Sky Survey galaxy data and halo data from up-to-date N-body simulations within the Lambda CDM framework we construct a semi-empirical catalog (SEC) of early-type galaxy-halo systems by making a self-consistent bivariate statistical match of stellar mass (M-*) and velocity dispersion (sigma) with halo virial mass (M-vir) as demonstrated here for the first time. We then assign stellar mass profile and velocity dispersion profile parameters to each system in the SEC using their observed correlations with M-* and sigma. Simultaneously, we solve for dark matter density profile of each halo using the spherical Jeans equation. The resulting dark matter density profiles deviate in general from the dissipationless profile of Navarro-Frenk-White or Einasto and their mean inner density slope and concentration vary systematically with M-vir. Statistical tests of the distribution of profiles at fixed M-vir rule out the null hypothesis that it follows the distribution predicted by dissipationless N-body simulations for M-vir less than or similar to 10(13.5-14.5) M-circle dot. These dark matter profiles imply that dark matter density is, on average, enhanced significantly in the inner region of halos with M-vir less than or similar to 10(13.5-14.5) M-circle dot supporting halo contraction. The main characteristics of halo contraction are: (1) the mean dark matter density within the effective radius has increased by a factor varying systematically up to approximate to 3-4 at M-vir = 10(12) M-circle dot, and (2) the inner density slope has a mean of approximate to 1.3 with rho(dm)(r) proportional to r(-alpha) and a halo-to-halo rms scatter of rms(alpha) similar to 0.4-0.5 for 10(12) M-circle dot less than or similar to M-vir less than or similar to 10(13-14) M-circle dot steeper than the NFW profile (alpha = 1). Based on our results we predict that halos of nearby elliptical and lenticular galaxies can, in principle, be promising targets for gamma-ray emission from dark matter annihilation. C1 [Chae, Kyu-Hyun] Sejong Univ, Dept Astron & Space Sci, Seoul 143747, South Korea. [Chae, Kyu-Hyun; Frieman, Joshua A.] Fermilab Natl Accelerator Lab, Ctr Particle Astrophys, Batavia, IL 60510 USA. [Kravtsov, Andrey V.; Frieman, Joshua A.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Kravtsov, Andrey V.; Frieman, Joshua A.] Univ Chicago, Dept Astron & Astrophys, Chicago, IL 60637 USA. [Bernardi, Mariangela] Univ Penn, Dept Phys & Astron, Philadelphia, PA 19104 USA. RP Chae, KH (reprint author), Sejong Univ, Dept Astron & Space Sci, 98 Gunja Dong, Seoul 143747, South Korea. EM chae@sejong.ac.kr; andrey@oddjob.uchicago.edu; frieman@fnal.gov; bernardm@physics.upenn.edu FU NSF [AST-0708154]; Kavli Institute for Cosmological Physics at the University of Chicago through the NSF [PHY-0551142, PHY-1125897]; Kavli Foundation; NASA [ADP/NNX09AD02G] FX We would like to thank Dan Hooper for conversations and comments on the draft and Anatoly Klypin for making outputs from the Bolshoi and Multidark simulations available to us. We would also like to thank the anonymous referees for useful suggestions, Aaron Dutton and Michele Cappellari for comments/discussions on stellar IMFs. KHC is grateful for the sabbatical leave (March 2010 January 2011) at Fermilab Center for Particle Astrophysics where significant parts of this work were carried out. He thanks in particular Albert Stebbins and Craig Hogan at FCPA for their encouragements. He also thanks In-Taek Gong at Sejong University for his assistance in preparing a figure. AVK was supported in part by the NSF grant AST-0708154, and by the Kavli Institute for Cosmological Physics at the University of Chicago through the NSF grant PHY-0551142 and PHY-1125897 and an endowment from the Kavli Foundation. MB is grateful for partial support provided by NASA grant ADP/NNX09AD02G. NR 84 TC 0 Z9 0 U1 0 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1475-7516 J9 J COSMOL ASTROPART P JI J. Cosmol. Astropart. Phys. PD NOV PY 2012 IS 11 DI 10.1088/1475-7516/2012/11/004 PG 42 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 033WW UT WOS:000310833100004 ER PT J AU Das, S de Putter, R Linder, EV Nakajima, R AF Das, Sudeep de Putter, Roland Linder, Eric V. Nakajima, Reiko TI Weak lensing cosmology beyond Lambda CDM SO JOURNAL OF COSMOLOGY AND ASTROPARTICLE PHYSICS LA English DT Article DE dark energy experiments; cosmological parameters from LSS; weak gravitational lensing; dark energy theory ID MATTER POWER SPECTRUM; COSMIC SHEAR; DARK ENERGY; PHOTOMETRIC REDSHIFTS; INTRINSIC ALIGNMENTS; MODIFIED GRAVITY; REQUIREMENTS; IMPACT; MODEL; CALIBRATION AB Weak gravitational lensing is one of the key probes of the cosmological model, dark energy, and dark matter, providing insight into both the cosmic expansion history and large scale structure growth history. Taking into account a broad spectrum of physics affecting growth - dynamical dark energy, extended gravity, neutrino masses, and spatial curvature - we analyze the cosmological constraints. Similarly we consider the effects of a range of systematic uncertainties, in shear measurement, photometric redshifts, intrinsic alignments, and the nonlinear power spectrum, on cosmological parameter extraction. We also investigate, and provide fitting formulas tor, the influence of survey parameters such as redshift depth, galaxy number densities, and sky area on the cosmological constraints in the beyond-ACDM parameter space. Finally, we examine the robustness of results for different fiducial cosmologies. C1 [Das, Sudeep; Linder, Eric V.; Nakajima, Reiko] Univ Calif Berkeley, Berkeley Ctr Cosmol Phys, Berkeley, CA 94720 USA. [de Putter, Roland] Univ Valencia, IFIC, CSIC, Valencia, Spain. [de Putter, Roland] Inst Ciencies Cosmos, Barcelona, Spain. [Linder, Eric V.; Nakajima, Reiko] Ewha Womans Univ, Inst Early Universe, Seoul, South Korea. [Linder, Eric V.; Nakajima, Reiko] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Linder, Eric V.; Nakajima, Reiko] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Nakajima, Reiko] Univ Bonn, Argelander Inst Astron, D-53121 Bonn, Germany. [Das, Sudeep] Argonne Natl Lab, Div High Energy Phys, Lemont, IL 60439 USA. RP Das, S (reprint author), Univ Calif Berkeley, Berkeley Ctr Cosmol Phys, Berkeley, CA 94720 USA. EM sdas@hep.anl.gov; rdeputter@icc.ub.edu; evlinder@lbl.gov; reiko@astro.uni-bonn.de FU Office of Science, Office of High Energy Physics, of the U.S. Department of Energy [DE-AC02-05CH11231]; World Class University grant through the National Research Foundation [R32-2008-000-10130-0]; Ministry of Education, Science and Technology of Korea; NASA LTSA grant [NNG04GC90G] FX We thank Dragan Huterer for useful discussions and Adam Bruce for crosschecks and creating the code GUI. This work has been supported in part by the Director, Office of Science, Office of High Energy Physics, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231, and also by the World Class University grant R32-2008-000-10130-0 through the National Research Foundation, Ministry of Education, Science and Technology of Korea (EL,RN). RN acknowledges partial support by NASA LTSA grant NNG04GC90G. NR 55 TC 0 Z9 0 U1 0 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1475-7516 J9 J COSMOL ASTROPART P JI J. Cosmol. Astropart. Phys. PD NOV PY 2012 IS 11 DI 10.1088/1475-7516/2012/11/011 PG 23 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 033WW UT WOS:000310833100011 ER PT J AU Franc, J Belas, E Bugar, M Hlidek, P Grill, R Yang, G Cavallini, A Fraboni, B Castaldini, A Assali, S AF Franc, J. Belas, E. Bugar, M. Hlidek, P. Grill, R. Yang, G. Cavallini, A. Fraboni, B. Castaldini, A. Assali, S. TI Semi insulating CdTe:Cl after elimination of inclusions and precipitates by post grown annealing SO JOURNAL OF INSTRUMENTATION LA English DT Article; Proceedings Paper CT 14th International Workshop on Radiation Imaging Detectors CY JUL 01-05, 2012 CL Figueira da Foz, PORTUGAL DE Solid state detectors; Charge transport and multiplication in solid media; Materials for solid-state detectors ID CL; CRYSTALS AB We present in this contribution results of two-step annealing, when the CdTe:Cl doped samples are at first annealed under Cd overpressure to remove inclusions and the re-annealed under Te overpressure to restore the high resistivity state. Investigation of samples after Cd rich annealing by infrared microscope has proven, that all inclusions are removed. Also Te nano precipitates were strongly influenced by the annealing process. The resistivity of the samples after Te-rich annealing was restored to values (similar to 10(8)-10(9) Omega cm). We observed, however, decrease of mobility-lifetime product of electrons from 10(-3)cm(2)/Vs to 10(-4)cm(2)/Vs. In order to understand the reason of this decrease we performed a study of point defects before and after annealing by thermoelectric effect spectroscopy. It shows a decrease of concentrations of most deep levels after two-step annealing. This behavior is completely different compared to past annealing studies, where concentration of deep levels strongly increased after annealing. The only level with an increased concentration in the current study is the midgap level (E similar to 0.8 eV). At the same time we observed increase of micro-twins in the samples investigated by transmission electron microscopy. The decrease of charge collection efficiency after two-step annealing may be therefore connected with re-arrangement of near midgap levels due to increase of concentrations of structure defects (micro twins, dislocations) that accumulate in their surroundings point defects with energy similar to 0.75 eV. C1 [Franc, J.; Belas, E.; Bugar, M.; Hlidek, P.; Grill, R.] Charles Univ Prague, Inst Phys, MFF, Prague 2, Czech Republic. [Yang, G.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Cavallini, A.; Fraboni, B.; Castaldini, A.; Assali, S.] Univ Bologna, Dept Phys, I-40126 Bologna, Italy. RP Franc, J (reprint author), Charles Univ Prague, Inst Phys, MFF, Ke Karlovu 5, Prague 2, Czech Republic. EM franc@karlov.mff.cuni.cz RI Grill, Roman/A-2109-2008; Franc, Jan/C-3802-2017 OI Grill, Roman/0000-0002-4615-8909; Franc, Jan/0000-0002-9493-3973 NR 7 TC 2 Z9 2 U1 1 U2 16 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD NOV PY 2012 VL 7 AR C11001 DI 10.1088/1748-0221/7/11/C11001 PG 5 WC Instruments & Instrumentation SC Instruments & Instrumentation GA 033XR UT WOS:000310835200001 ER PT J AU Kutsaev, SV Kelly, MP Ostroumov, PN AF Kutsaev, S. V. Kelly, M. P. Ostroumov, P. N. TI Design of RF power coupler for superconducting cavities SO JOURNAL OF INSTRUMENTATION LA English DT Article DE Accelerator Subsystems and Technologies; Acceleration cavities and magnets superconducting; (high-temperature superconductor; radiation hardened magnets; normal-conducting; permanent magnet devices; wigglers and undulators) AB A new power coupler has been designed and is being prototyped by Argonne National Laboratory (ANL) for use with any of the ANL proposed superconducting (SC) half-or quarter-wave cavities for SARAF [1] and Project-X [2]. The 50 Ohm coaxial capacitive coupler is required to operate in the CW regime with up to 15kW of forward power and under any condition for the reflected power. A key feature is a moveable copper plated stainless steel bellows which will permit up to 3 cm of axial stroke and adjustment of the external quality factor by roughly one order of magnitude in the range of 10(5) to 10(6). The mechanical and vacuum design includes two ceramic windows, one operating at room temperature and another at 70 Kelvin. The two window design allows the portion of the coupler assembled onto the SC cavity in the clean room to be compact and readily cleanable. Other design features include thermal intercepts to provide a large margin for RF heating and a mechanical guide assembly to operate cold and under vacuum with high reliability. C1 [Kutsaev, S. V.; Kelly, M. P.; Ostroumov, P. N.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. RP Kutsaev, SV (reprint author), Argonne Natl Lab, Div Phys, 9700 S Cass Ave, Argonne, IL 60439 USA. EM s_kutsaev@mail.ru OI Kutsaev, Sergey/0000-0003-4996-2545 FU U.S. Department of Energy, Office of High Energy Physics [DE-AC02-76CH03000]; Office of Nuclear Physics [DEAC02-06CH11357] FX This work was supported by the U.S. Department of Energy, Office of High Energy Physics, under Contract DE-AC02-76CH03000 and the Office of Nuclear Physics, under Contract No. DEAC02-06CH11357. NR 18 TC 0 Z9 0 U1 1 U2 8 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD NOV PY 2012 VL 7 AR P11004 DI 10.1088/1748-0221/7/11/P11004 PG 18 WC Instruments & Instrumentation SC Instruments & Instrumentation GA 033XR UT WOS:000310835200006 ER PT J AU Hu, JP Hawes, C AF Hu, Jianping Hawes, Chris TI Recent Advances in Plant Organelle Dynamics SO JOURNAL OF INTEGRATIVE PLANT BIOLOGY LA English DT Editorial Material C1 [Hu, Jianping] Michigan State Univ, MSU DOE Plant Res Lab, E Lansing, MI 48824 USA. [Hu, Jianping] Michigan State Univ, Dept Plant Biol, E Lansing, MI 48824 USA. [Hawes, Chris] Oxford Brookes Univ, Dept Biol & Med Sci, Oxford OX3 0BP, England. RP Hu, JP (reprint author), Michigan State Univ, MSU DOE Plant Res Lab, E Lansing, MI 48824 USA. NR 7 TC 1 Z9 1 U1 0 U2 7 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1672-9072 J9 J INTEGR PLANT BIOL JI J. Integr. Plant Biol. PD NOV PY 2012 VL 54 IS 11 SI SI BP 838 EP 839 DI 10.1111/j.1744-7909.2012.01181.x PG 2 WC Biochemistry & Molecular Biology; Plant Sciences SC Biochemistry & Molecular Biology; Plant Sciences GA 036UN UT WOS:000311057400002 PM 23066711 ER PT J AU Aung, K Hu, JP AF Aung, Kyaw Hu, Jianping TI Differential Roles of Arabidopsis Dynamin-Related Proteins DRP3A, DRP3B, and DRP5B in Organelle Division SO JOURNAL OF INTEGRATIVE PLANT BIOLOGY LA English DT Article DE Arabidopsis; dynamin-related protein; mitochondria ID MITOCHONDRIAL DIVISION; CHLOROPLAST DIVISION; PLANT DEVELOPMENT; CRYSTAL-STRUCTURE; PLASTID DIVISION; FISSION; PROLIFERATION; ENDOCYTOSIS; DRP1A; MORPHOGENESIS AB Dynamin-related proteins (DRPs) are key components of the organelle division machineries, functioning as molecular scissors during the fission process. In Arabidopsis, DRP3A and DRP3B are shared by peroxisomal and mitochondrial division, whereas the structurally-distinct DRP5B (ARC5) protein is involved in the division of chloroplasts and peroxisomes. Here, we further investigated the roles of DRP3A, DRP3B, and DRP5B in organelle division and plant development. Despite DRP5B's lack of stable association with mitochondria, drp5B mutants show defects in mitochondrial division. The drp3A-2 drp3B-2 drp5B-2 triple mutant exhibits enhanced mitochondrial division phenotypes over drp3A-2 drp3B-2, but its peroxisomal morphology and plant growth phenotypes resemble those of the double mutant. We further demonstrated that DRP3A and DRP3B form a supercomplex in vivo, in which DRP3A is the major component, yet DRP5B is not a constituent of this complex. We thus conclude that DRP5B participates in the division of three types of organelles in Arabidopsis, acting independently of the DRP3 complex. Our findings will help elucidate the precise composition of the DRP3 complex at organelle division sites, and will be instrumental to studies aimed at understanding how the same protein mediates the morphogenesis of distinct organelles that are linked by metabolism. C1 [Hu, Jianping] Michigan State Univ, MSU DOE Plant Res Lab, E Lansing, MI 48824 USA. Michigan State Univ, Dept Plant Biol, E Lansing, MI 48824 USA. RP Aung, K (reprint author), Michigan State Univ, MSU DOE Plant Res Lab, E Lansing, MI 48824 USA. EM huji@msu.edu FU National Science Foundation Arabidopsis program [MCB 0618335]; Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy [DE-FG02-91ER20021] FX We thank Kathy Osteryoung (Michigan State University) for seeds of arc5 (drp5B-1), arc6, and the ftsZ2 double mutant. This work was supported by grants from the National Science Foundation Arabidopsis 2010 program (MCB 0618335) and the Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy (DE-FG02-91ER20021) to J.H. NR 43 TC 7 Z9 7 U1 0 U2 16 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1672-9072 J9 J INTEGR PLANT BIOL JI J. Integr. Plant Biol. PD NOV PY 2012 VL 54 IS 11 SI SI BP 921 EP 931 DI 10.1111/j.1744-7909.2012.01174.x PG 11 WC Biochemistry & Molecular Biology; Plant Sciences SC Biochemistry & Molecular Biology; Plant Sciences GA 036UN UT WOS:000311057400001 PM 23046048 ER PT J AU Parson, WB Koeniger, SL Johnson, RW Erickson, J Tian, Y Stedman, C Schwartz, A Tarcsa, E Cole, R Van Berkel, GJ AF Parson, Whitney B. Koeniger, Stormy L. Johnson, Robert W. Erickson, Jamie Tian, Yu Stedman, Christopher Schwartz, Annette Tarcsa, Edit Cole, Roderic Van Berkel, Gary J. TI Analysis of chloroquine and metabolites directly from whole-body animal tissue sections by liquid extraction surface analysis (LESA) and tandem mass spectrometry SO JOURNAL OF MASS SPECTROMETRY LA English DT Article DE tissue analysis; imaging; mass spectrometry; chloroquine; surface sampling; LESA ID DRUG DISCOVERY; MALDI-MS; AUTORADIOGRAPHY; STANDARDIZATION; UTILITY; SYSTEM; SPACE; ADME; RATS AB The rapid and direct analysis of the amount and spatial distribution of exogenous chloroquine (CHQ) and CHQ metabolites from tissue sections by liquid extraction surface sampling analysis coupled with tandem mass spectrometry (LESA-MS/MS) was demonstrated. LESA-MS/MS results compared well with previously published CHQ quantification data collected by organ excision, extraction and fluorescent detection. The ability to directly sample and analyze spatially resolved exogenous molecules from tissue sections with minimal sample preparation and analytical method development has the potential to facilitate the assessment of target tissue penetration of pharmaceutical compounds, to establish pharmacokinetic/pharmacodynamic relationships, and to complement established pharmacokinetic methods used in the drug discovery process during tissue distribution assessment. Copyright (c) 2012 John Wiley & Sons, Ltd. C1 [Parson, Whitney B.; Van Berkel, Gary J.] Oak Ridge Natl Lab, Div Chem Sci, Organ & Biol Mass Spectrometry Grp, Oak Ridge, TN 37831 USA. [Koeniger, Stormy L.; Johnson, Robert W.] Abbott Labs, GPRD, Adv Technol, Abbott Pk, IL 60064 USA. [Erickson, Jamie; Tian, Yu; Stedman, Christopher; Schwartz, Annette; Tarcsa, Edit; Cole, Roderic] Abbott Labs, Drug Metab & Pharmacokinet, Worcester, MA USA. RP Van Berkel, GJ (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Organ & Biol Mass Spectrometry Grp, Oak Ridge, TN 37831 USA. EM vanberkelgj@ornl.gov FU U.S. Government [DE-AC05-00OR22725]; Abbott Laboratories, Chicago, IL; Abbott Laboratories, Worcester, MA FX This manuscript has been authored by a contractor of the U.S. Government under contract DE-AC05-00OR22725. Accordingly, the U. S. Government retains a paid-up, nonexclusive, irrevocable, worldwide license to publish or reproduce the published form of this contribution, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, or allow others to do so, for U. S. Government purposes.; Work at Oak Ridge National laboratory (ORNL) was funded by a Work for Others Agreement with Abbott Laboratories, Chicago, IL and Worcester, MA. NR 48 TC 16 Z9 17 U1 4 U2 40 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1076-5174 J9 J MASS SPECTROM JI J. Mass Spectrom. PD NOV PY 2012 VL 47 IS 11 BP 1420 EP 1428 DI 10.1002/jms.3068 PG 9 WC Biochemical Research Methods; Chemistry, Analytical; Spectroscopy SC Biochemistry & Molecular Biology; Chemistry; Spectroscopy GA 037HP UT WOS:000311093400005 PM 23147817 ER PT J AU Deri, Y Chapman, J Biegon, A AF Deri, Y. Chapman, J. Biegon, A. TI Time, sex and region-dependent neuroinflammation in cortex and hippocampus of mice with Experimental Autoimmune Encephalo- myelitis (EAE) SO JOURNAL OF MOLECULAR NEUROSCIENCE LA English DT Meeting Abstract CT 20th Annual Meeting of the Israel-Society-for-Neuroscience CY DEC 11-13, 2011 CL Eilat, ISRAEL SP Israel Soc Neurosci C1 [Deri, Y.] Tel Aviv Univ, Joseph Sagol Neurosci Ctr, Chaim Sheba Med Ctr, Tel Aviv, Israel. [Deri, Y.; Chapman, J.] Tel Aviv Univ, Sackler Fac Med, Tel Aviv, Israel. [Chapman, J.] Chaim Sheba Med Ctr, Dept Neurol, Tel Hashomer, Israel. [Biegon, A.] Brookhaven Natl Lab, Upton, NY 11973 USA. RI Chapman, Joab/E-4598-2010 NR 0 TC 0 Z9 0 U1 0 U2 0 PU HUMANA PRESS INC PI TOTOWA PA 999 RIVERVIEW DRIVE SUITE 208, TOTOWA, NJ 07512 USA SN 0895-8696 J9 J MOL NEUROSCI JI J. Mol. Neurosci. PD NOV PY 2012 VL 48 SU 1 BP S25 EP S26 PG 2 WC Biochemistry & Molecular Biology; Neurosciences SC Biochemistry & Molecular Biology; Neurosciences & Neurology GA 030BC UT WOS:000310541600058 ER PT J AU Livny-Ezer, A Weiser, M Kushnir, T Harnof, S Tomasi, D Biegon, A AF Livny-Ezer, A. Weiser, M. Kushnir, T. Harnof, S. Tomasi, D. Biegon, A. TI Effect of increased working memory load on brain activation patterns in subjects with traumatic brain injury and controls: an fMRI study SO JOURNAL OF MOLECULAR NEUROSCIENCE LA English DT Meeting Abstract CT 20th Annual Meeting of the Israel-Society-for-Neuroscience CY DEC 11-13, 2011 CL Eilat, ISRAEL SP Israel Soc Neurosci C1 [Livny-Ezer, A.] Chaim Sheba Med Ctr, J Sagol Neurosci Ctr, IL-52621 Tel Hashomer, Israel. [Livny-Ezer, A.; Weiser, M.; Kushnir, T.] Tel Aviv Univ, Sackler Fac Med, Tel Aviv, Israel. [Weiser, M.] Chaim Sheba Med Ctr, Dept Psychiat, IL-52621 Tel Hashomer, Israel. [Kushnir, T.] Chaim Sheba Med Ctr, Dept Diagnost Imaging, MRI Unit, IL-52621 Tel Hashomer, Israel. [Harnof, S.] Chaim Sheba Med Ctr, Dept Neurosurg, IL-52621 Tel Hashomer, Israel. [Tomasi, D.; Biegon, A.] Brookhaven Natl Lab, Upton, NY 11973 USA. RI Tomasi, Dardo/J-2127-2015 NR 0 TC 0 Z9 0 U1 0 U2 2 PU HUMANA PRESS INC PI TOTOWA PA 999 RIVERVIEW DRIVE SUITE 208, TOTOWA, NJ 07512 USA SN 0895-8696 J9 J MOL NEUROSCI JI J. Mol. Neurosci. PD NOV PY 2012 VL 48 SU 1 BP S72 EP S72 PG 1 WC Biochemistry & Molecular Biology; Neurosciences SC Biochemistry & Molecular Biology; Neurosciences & Neurology GA 030BC UT WOS:000310541600184 ER PT J AU Livny-Ezer, A Weiser, M Kushnir, T Harnof, S Tomasi, D Biegon, A AF Livny-Ezer, A. Weiser, M. Kushnir, T. Harnof, S. Tomasi, D. Biegon, A. TI Effect of intelligence quotient (IQ) on brain activation patterns in subjects performing a working memory task: an fMRI study SO JOURNAL OF MOLECULAR NEUROSCIENCE LA English DT Meeting Abstract CT 20th Annual Meeting of the Israel-Society-for-Neuroscience CY DEC 11-13, 2011 CL Eilat, ISRAEL SP Israel Soc Neurosci C1 [Livny-Ezer, A.] Chaim Sheba Med Ctr, J Sagol Neurosci Ctr, IL-52621 Tel Hashomer, Israel. [Livny-Ezer, A.; Weiser, M.; Kushnir, T.] Tel Aviv Univ, Sackler Fac Med, Tel Aviv, Israel. [Weiser, M.] Chaim Sheba Med Ctr, Dept Psychiat, IL-52621 Tel Hashomer, Israel. [Kushnir, T.] Chaim Sheba Med Ctr, Dept Diagnost Imaging, MRI Unit, IL-52621 Tel Hashomer, Israel. [Harnof, S.] Chaim Sheba Med Ctr, Dept Neurosurg, IL-52621 Tel Hashomer, Israel. [Tomasi, D.; Biegon, A.] Brookhaven Natl Lab, Upton, NY 11973 USA. RI Tomasi, Dardo/J-2127-2015 NR 0 TC 0 Z9 0 U1 1 U2 3 PU HUMANA PRESS INC PI TOTOWA PA 999 RIVERVIEW DRIVE SUITE 208, TOTOWA, NJ 07512 USA SN 0895-8696 J9 J MOL NEUROSCI JI J. Mol. Neurosci. PD NOV PY 2012 VL 48 SU 1 BP S71 EP S72 PG 2 WC Biochemistry & Molecular Biology; Neurosciences SC Biochemistry & Molecular Biology; Neurosciences & Neurology GA 030BC UT WOS:000310541600183 ER PT J AU Zaltsman, SL Alexandrovich, AG Yaka, R Shohami, E Biegon, A AF Zaltsman, Liraz S. Alexandrovich, A. G. Yaka, R. Shohami, E. Biegon, A. TI Activation of glutamate receptors with single dose of DCS reverses long-term cognitive deficits in a mouse model of neuroinflammation SO JOURNAL OF MOLECULAR NEUROSCIENCE LA English DT Meeting Abstract CT 20th Annual Meeting of the Israel-Society-for-Neuroscience CY DEC 11-13, 2011 CL Eilat, ISRAEL SP Israel Soc Neurosci C1 [Zaltsman, Liraz S.; Alexandrovich, A. G.; Yaka, R.; Shohami, E.] Hebrew Univ Jerusalem, Dept Pharmacol, Jerusalem, Israel. [Biegon, A.] Brookhaven Natl Lab, Upton, NY 11973 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU HUMANA PRESS INC PI TOTOWA PA 999 RIVERVIEW DRIVE SUITE 208, TOTOWA, NJ 07512 USA SN 0895-8696 J9 J MOL NEUROSCI JI J. Mol. Neurosci. PD NOV PY 2012 VL 48 SU 1 BP S70 EP S71 PG 2 WC Biochemistry & Molecular Biology; Neurosciences SC Biochemistry & Molecular Biology; Neurosciences & Neurology GA 030BC UT WOS:000310541600180 ER PT J AU Li, N Shi, SS Tang, AH Wu, YF AF Li, Na Shi, Shusu Tang, Aihong Wu, Yuanfang TI The study of non-collectivity by the forward-backward multiplicity correlation function SO JOURNAL OF PHYSICS G-NUCLEAR AND PARTICLE PHYSICS LA English DT Article ID HEAVY-ION COLLISIONS; MATTER AB We propose a forward-backward multiplicity correlation function C-FB(N), which is experimentally accessible, to measure the non-collectivity contribution. It is found that the function is sensitive to both the jet contribution and small number statistics. We point out that the effect of the latter is also involved in the previous studies of the forward-backward elliptic correlation function but was misinterpreted as a contribution from jets. We study the C-FB(N) in Au+Au collision at root S-NN = 200 GeV with a multiphase transport model (AMPT). The result shows that the estimated jet contribution is much smaller than in the previous study due to the finite number statistics which has not been noticed before. The connection between this study and the forward-backward elliptic correlation function is also discussed. C1 [Li, Na] Huazhong Univ Sci & Technol, Dept Phys, Wuhan 430074, Peoples R China. [Shi, Shusu; Wu, Yuanfang] Cent China Normal Univ HZNU, Inst Particle Phys, Wuhan 430079, Peoples R China. [Tang, Aihong] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Li, N (reprint author), Huazhong Univ Sci & Technol, Dept Phys, Wuhan 430074, Peoples R China. EM nli@mail.hust.edu.cn; sss@iopp.ccnu.edu.cn FU Huazhong University of Science and Technology Foundation [2011QN195]; National Natural Science Foundation of China [11147196, 11105060, 10835005]; Office of Nuclear Physics, US Department of Energy [DE-AC02-98CH10886, DE-FG02-89ER40531] FX The authors thank L X Han, J Liao and G Wang for useful discussions. The work was supported in part by Huazhong University of Science and Technology Foundation under grant no. 2011QN195, the National Natural Science Foundation of China under grant nos 11147196, 11105060 and 10835005, and by the Office of Nuclear Physics, US Department of Energy under grants DE-AC02-98CH10886 and DE-FG02-89ER40531. NR 24 TC 5 Z9 5 U1 1 U2 4 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0954-3899 J9 J PHYS G NUCL PARTIC JI J. Phys. G-Nucl. Part. Phys. PD NOV PY 2012 VL 39 IS 11 AR 115105 DI 10.1088/0954-3899/39/11/115105 PG 8 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA 030HX UT WOS:000310562900007 ER PT J AU Ho, CK Khalsa, SS AF Ho, Clifford K. Khalsa, Siri S. TI A Photographic Flux Mapping Method for Concentrating Solar Collectors and Receivers SO JOURNAL OF SOLAR ENERGY ENGINEERING-TRANSACTIONS OF THE ASME LA English DT Article DE flux map; concentrating solar; receiver; irradiance; heliostat; collector ID DISH AB A new method is described to determine irradiance distributions on receivers and targets from heliostats or other collectors for concentrating solar power applications. The method uses a digital camera, and, unlike previous beam characterization systems, it does not require additional sensors, calorimeters, or flux gauges on the receiver or target. In addition, spillage can exist and can also be measured (the beam does not need to be contained within the target). The only additional information required besides the images recorded from the digital camera is the direct normal irradiance and the reflectivity of the receiver. Methods are described to calculate either an average reflectivity or a reflectivity distribution for the receiver using the digital camera. The novel feature of this new photographic flux (PHLUX) mapping method is the use of recorded images of the sun to scale both the magnitude of each pixel value and the subtended angle of each pixel. A test was performed to evaluate the PHLUX method using a heliostat beam on the central receiver tower at the National Solar Thermal Test Facility in Albuquerque, NM. Results showed that the PHLUX method was capable of producing an accurate flux map of the heliostat beam on a Lambertian surface with a relative error in the peak flux of similar to 2% when the filter attenuation factors and effective receiver reflectivity were well characterized. Total relative errors associated with the measured irradiance using the PHLUX method can be up to 20%-40%, depending on various error sources identified in the paper, namely, uncertainty in receiver reflectivity and filter attenuation. [DOI: 10.1115/1.4006892] C1 [Ho, Clifford K.; Khalsa, Siri S.] Sandia Natl Labs, Concentrating Solar Technol Dept, Albuquerque, NM 87185 USA. RP Ho, CK (reprint author), Sandia Natl Labs, Concentrating Solar Technol Dept, POB 5800, Albuquerque, NM 87185 USA. EM ckho@sandia.gov FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. NR 15 TC 9 Z9 11 U1 2 U2 20 PU ASME-AMER SOC MECHANICAL ENG PI NEW YORK PA THREE PARK AVE, NEW YORK, NY 10016-5990 USA SN 0199-6231 J9 J SOL ENERG-T ASME JI J. Sol. Energy Eng. Trans.-ASME PD NOV PY 2012 VL 134 IS 4 AR 041004 DI 10.1115/1.4006892 PG 8 WC Energy & Fuels; Engineering, Mechanical SC Energy & Fuels; Engineering GA 034EJ UT WOS:000310852800005 ER PT J AU Zhu, GD Lewandowski, A AF Zhu, Guangdong Lewandowski, Allan TI A New Optical Evaluation Approach for Parabolic Trough Collectors: First-Principle OPTical Intercept Calculation SO JOURNAL OF SOLAR ENERGY ENGINEERING-TRANSACTIONS OF THE ASME LA English DT Article DE parabolic trough; concentrating solar power; optical performance; optical analysis; intercept factor AB A new analytical method-First-principle OPTical Intercept Calculation (FirstOPTIC)-is presented here for optical evaluation of trough collectors. It employs first-principle optical treatment of collector optical error sources and derives analytical mathematical formulae to calculate the intercept factor of a trough collector. A suite of MATLAB code is developed for FirstOPTIC and validated against theoretical/numerical solutions and ray-tracing results. It is shown that FirstOPTIC can provide fast and accurate calculation of intercept factors of trough collectors. The method makes it possible to carry out fast evaluation of trough collectors for design purposes. The FirstOPTIC techniques and analysis may be naturally extended to other types of CSP technologies such as linear-Fresnel collectors and central-receiver towers. [DOI: 10.1115/1.4006963] C1 [Zhu, Guangdong; Lewandowski, Allan] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Zhu, GD (reprint author), Natl Renewable Energy Lab, MS 5202,15013 Denver W Pkwy, Golden, CO 80401 USA. EM Guangdong.Zhu@nrel.gov FU U.S. Department of Energy [DE-AC36-08GO28308]; National Renewable Energy Laboratory (NREL) FX This work was supported by the U.S. Department of Energy under Contract No. DE-AC36-08GO28308 with the National Renewable Energy Laboratory (NREL). The authors would like to thank the thermal systems group staff at NREL for providing their valuable feedbacks for this work. NR 22 TC 9 Z9 9 U1 0 U2 7 PU ASME-AMER SOC MECHANICAL ENG PI NEW YORK PA THREE PARK AVE, NEW YORK, NY 10016-5990 USA SN 0199-6231 J9 J SOL ENERG-T ASME JI J. Sol. Energy Eng. Trans.-ASME PD NOV PY 2012 VL 134 IS 4 AR 041005 DI 10.1115/1.4006963 PG 8 WC Energy & Fuels; Engineering, Mechanical SC Energy & Fuels; Engineering GA 034EJ UT WOS:000310852800006 ER PT J AU Satoh, Y Tajima, K Munekata, M Keasling, JD Lee, TS AF Satoh, Yasuharu Tajima, Kenji Munekata, Masanobu Keasling, Jay D. Lee, Taek Soon TI Engineering of L-tyrosine oxidation in Escherichia coli and microbial production of hydroxytyrosol SO METABOLIC ENGINEERING LA English DT Article DE Tyrosine hydroxylase; Tetrahydrobiopterin; Tetrahydromonapterin; Dopa decarboxylase; Hydroxytyrosol; Microbial production ID AMINO-ACID HYDROXYLASES; MICROBIOLOGICAL TRANSFORMATION; L-DOPA; TETRAHYDROBIOPTERIN; BIOSYNTHESIS; PURIFICATION; K-12; TETRAHYDROPTERIN; PHENYLALANINE; TRYPTOPHAN AB The hydroxylation of tyrosine is an important reaction in the biosynthesis of many natural products. The use of bacteria for this reaction has not been very successful due to either the over-oxidation to ortho-quinone when using tyrosinases from bacteria or plants, or the lack of the native cofactor, tetrahydrobiopterin (BH4), needed for the activity of tyrosine hydroxylases (TH). Here, we demonstrate that an Escherichia coli cofactor, tetrahydromonapterin (MH4), can be used as an alternative cofactor for TH in presence of the BH4 regeneration pathway, and tyrosine hydroxylation is performed without over-oxidation. We used this platform for biosynthesis of one of the most powerful antioxidants, hydroxytyrosol. An endogenous aromatic aldehyde oxidase was identified and knocked out to prevent formation of the side product, and this resulted in nearly exclusive production of hydroxytyrosol in engineered E. coli. Finally, hydroxytyrosol production from a simple sugar as a sole carbon source was demonstrated. Published by Elsevier Inc. C1 [Keasling, Jay D.; Lee, Taek Soon] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Satoh, Yasuharu; Keasling, Jay D.; Lee, Taek Soon] Joint BioEnergy Inst, Emeryville, CA 94608 USA. [Satoh, Yasuharu; Tajima, Kenji; Munekata, Masanobu] Hokkaido Univ, Fac Engn, Sapporo, Hokkaido 0608628, Japan. [Keasling, Jay D.; Lee, Taek Soon] Univ Calif Berkeley, Synthet Biol Engn Res Ctr, Berkeley, CA 94720 USA. [Keasling, Jay D.] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. [Keasling, Jay D.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. RP Lee, TS (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. EM tslee@lbl.gov RI Keasling, Jay/J-9162-2012; Satoh, Yasuharu/H-4174-2012; OI Keasling, Jay/0000-0003-4170-6088; Satoh, Yasuharu/0000-0001-6671-7758 FU Synthetic Biology Engineering Research Center (SynBERC) through National Science Foundation grant [BES-0439124]; Joint BioEnergy Institute [DE-AC02-05CH11231]; Global COE Program (Catalysis as the Basis for Innovation in materials science) from the Ministry of Education, Culture, Sports, Science, and Technology in Japan [B01] FX We thank Darmawi Juminaga, Edward Baidoo and Peter Benke from the Joint BioEnergy Institute for their valuable discussion and technical support. This work was supported by the Synthetic Biology Engineering Research Center (SynBERC) through National Science Foundation grant BES-0439124 and by the Joint BioEnergy Institute through contract DE-AC02-05CH11231 between Lawrence Berkeley National Laboratory and the US Department of Energy. YS was supported by the Global COE Program (Project No. B01: Catalysis as the Basis for Innovation in materials science) from the Ministry of Education, Culture, Sports, Science, and Technology in Japan. NR 45 TC 16 Z9 17 U1 7 U2 58 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 1096-7176 J9 METAB ENG JI Metab. Eng. PD NOV PY 2012 VL 14 IS 6 BP 603 EP 610 DI 10.1016/j.ymben.2012.08.002 PG 8 WC Biotechnology & Applied Microbiology SC Biotechnology & Applied Microbiology GA 035DW UT WOS:000310924400001 PM 22948011 ER PT J AU Zhang, FZ Ouellet, M Batth, TS Adams, PD Petzold, CJ Mukhopadhyay, A Keasling, JD AF Zhang, Fuzhong Ouellet, Mario Batth, Tanveer S. Adams, Paul D. Petzold, Christopher J. Mukhopadhyay, Aindrila Keasling, Jay D. TI Enhancing fatty acid production by the expression of the regulatory transcription factor FadR SO METABOLIC ENGINEERING LA English DT Article DE Fatty acid production; FadR; Global regulation; Metabolic engineering ID ESCHERICHIA-COLI; MICROBIAL-PRODUCTION; ACYL-COENZYME; DNA-BINDING; CHEMICALS; OVERPRODUCTION; BIOSYNTHESIS; METABOLISM; BIOFUELS; ALKANES AB Fatty acids are important precursors to biofuels. The Escherichia coli FadR is a transcription factor that regulates several processes in fatty acid biosynthesis, degradation, and membrane transport. By tuning the expression of FadR in an engineered E. coli host, we were able to increase fatty acid titer by 7.5-fold over our previously engineered fatty acid-producing strain, reaching 5.2 +/- 0.5 g/L and 73% of the theoretical yield. The mechanism by which FadR enhanced fatty acid yield was studied by whole genome transcriptional analysis (microarray) and targeted proteomics. Overexpression of FadR led to transcriptional changes for many genes, including genes involved in fatty acid pathways. The biggest transcriptional changes in fatty acid pathway genes included fabB, fabF, and accA. Overexpression of any of these genes alone did not result in a high yield comparable to fadR expression, indicating that FadR enhanced fatty acid production globally by tuning the expression levels of many genes to optimal levels. (C) 2012 Published by Elsevier Inc. C1 [Zhang, Fuzhong; Ouellet, Mario; Batth, Tanveer S.; Adams, Paul D.; Petzold, Christopher J.; Mukhopadhyay, Aindrila; Keasling, Jay D.] Joint BioEnergy Inst, Emeryville, CA 94608 USA. [Zhang, Fuzhong; Ouellet, Mario; Batth, Tanveer S.; Adams, Paul D.; Petzold, Christopher J.; Mukhopadhyay, Aindrila; Keasling, Jay D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Zhang, Fuzhong; Keasling, Jay D.] Univ Calif Berkeley, Calif Inst Quantitat Biosci, Berkeley, CA 94720 USA. [Zhang, Fuzhong; Keasling, Jay D.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Keasling, Jay D.] Univ Calif Berkeley, Synthet Biol Engn Res Ctr, Berkeley, CA 94720 USA. [Keasling, Jay D.] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. RP Keasling, JD (reprint author), Joint BioEnergy Inst, 5885 Hollis St, Emeryville, CA 94608 USA. EM keasling@berkeley.edu RI Adams, Paul/A-1977-2013; Keasling, Jay/J-9162-2012 OI Adams, Paul/0000-0001-9333-8219; Keasling, Jay/0000-0003-4170-6088 FU Synthetic Biology Engineering Research Center; National Science Foundation [0540879]; Joint BioEnergy Institute; U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research [DE-AC02-05CH11231]; Natural Sciences and Engineering Research Council of Canada; California Institute for Quantitative Biosciences FX The authors would like to thank Harry Beller and Ee-Been Goh for discussion and critical reading of the manuscript. This work was supported in part by the Synthetic Biology Engineering Research Center, which is funded by National Science Foundation Award no. 0540879, and by the Joint BioEnergy Institute, which is funded by the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research, through contract DE-AC02-05CH11231. F.Z. is supported by the Postdoctoral Fellowships Program of the Natural Sciences and Engineering Research Council of Canada and by the California Institute for Quantitative Biosciences. NR 31 TC 74 Z9 76 U1 7 U2 89 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 1096-7176 J9 METAB ENG JI Metab. Eng. PD NOV PY 2012 VL 14 IS 6 BP 653 EP 660 DI 10.1016/j.ymben.2012.08.009 PG 8 WC Biotechnology & Applied Microbiology SC Biotechnology & Applied Microbiology GA 035DW UT WOS:000310924400006 PM 23026122 ER PT J AU Agnew, DE Stevermer, AK Youngquist, JT Pfleger, BF AF Agnew, Daniel E. Stevermer, Amanda K. Youngquist, J. Tyler Pfleger, Brian F. TI Engineering Escherichia coli for production of C-12-C-14 polyhydroxyalkanoate from glucose SO METABOLIC ENGINEERING LA English DT Article DE E. coli; Thioesterase; Polyhydroxyalkanoate; Homopolymer; beta-oxidation; Dodecanoic acid ID CARRIER PROTEIN THIOESTERASE; BETA-OXIDATION PATHWAY; FATTY-ACIDS; PSEUDOMONAS-AERUGINOSA; LENGTH POLYHYDROXYALKANOATES; TAC PROMOTER; EXPRESSION; BIOSYNTHESIS; GENE; PUTIDA AB Demand for sustainable materials motivates the development of microorganisms capable of synthesizing products from renewable substrates. A challenge to commercial production of polyhydroxyalkanoates (PHA), microbially derived polyesters, is engineering metabolic pathways to produce a polymer with the desired monomer composition from an unrelated and renewable source. Here, we demonstrate a metabolic pathway for converting glucose into medium-chain-length (mcl)-PHA composed primarily of 3-hydroxydodecanoate monomers. This pathway combines fatty acid biosynthesis, an acyl-ACP thioesterase to generate desired C-12 and C-14 fatty acids, beta-oxidation for conversion of fatty acids to (R)-3-hydroxyacyl-CoAs, and a PHA polymerase. A key finding is that Escherichiacoli expresses multiple copies of enzymes involved in beta-oxidation under aerobic conditions. To produce polyhydroxydodecanoate, an acyl-ACP thioesterase (BTE), an enoyl-CoA hydratase (phaJ3), and mcl-PHA polymerase (phaC2) were overexpressed in E. coli Delta fadRABIJ. Yields were improved through expression of an acyl-CoA synthetase resulting in production over 15% CDW the highest reported production of mcl-PHA of a defined composition from an unrelated carbon source. (C) 2012 Elsevier Inc. All rights reserved. C1 [Agnew, Daniel E.; Stevermer, Amanda K.; Youngquist, J. Tyler; Pfleger, Brian F.] Univ Wisconsin, Dept Chem & Biol Engn, Madison, WI 53706 USA. [Youngquist, J. Tyler; Pfleger, Brian F.] Univ Wisconsin, Great Lakes Bioenergy Res Ctr, Madison, WI 53706 USA. RP Pfleger, BF (reprint author), Univ Wisconsin, Dept Chem & Biol Engn, 3629 Engn Hall,1415 Engn Dr, Madison, WI 53706 USA. EM pfleger@engr.wisc.edu FU DOE Great Lakes Bioenergy Research Center (DOE BER Office of Science) [DE-FC02-07ER64494]; Wisconsin Alumni Research Foundation; National Institutes of Health Biotechnology Training Program Fellowship [NIH 5 T32 GM08349]; National Science Foundation [NSF CHE-9208463, NSF CHE-0342998] FX This work was funded by the DOE Great Lakes Bioenergy Research Center (DOE BER Office of Science DE-FC02-07ER64494), and the Wisconsin Alumni Research Foundation. Daniel E. Agnew is the recipient of a National Institutes of Health Biotechnology Training Program Fellowship (NIH 5 T32 GM08349).; This material is based upon work supported by the National Science Foundation under Grant Nos. NSF CHE-9208463 and NSF CHE-0342998. NR 42 TC 27 Z9 28 U1 4 U2 41 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 1096-7176 J9 METAB ENG JI Metab. Eng. PD NOV PY 2012 VL 14 IS 6 BP 705 EP 713 DI 10.1016/j.ymben.2012.08.003 PG 9 WC Biotechnology & Applied Microbiology SC Biotechnology & Applied Microbiology GA 035DW UT WOS:000310924400010 PM 23141473 ER PT J AU Piazza, G Felmetsger, V Muralt, P Olsson, RH Ruby, R AF Piazza, Gianluca Felmetsger, Valeriy Muralt, Paul Olsson, Roy H., III Ruby, Richard TI Piezoelectric aluminum nitride thin films for microelectromechanical systems SO MRS BULLETIN LA English DT Article ID BULK ACOUSTIC RESONATORS; MEMS; TECHNOLOGY; FILTERS; STRESS AB This article reports on the state-of-the-art of the development of aluminum nitride (AlN) thin-film microelectromechanical systems (MEMS) with particular emphasis on acoustic devices for radio frequency (RF) signal processing. Examples of resonant devices are reviewed to highlight the capabilities of AlN as an integrated circuit compatible material for the implementation of RF filters and oscillators. The commercial success of thin-film bulk acoustic resonators is presented to show how AlN has de facto become an industrial standard for the synthesis of high performance duplexers. The article also reports on the development of a new class of AlN acoustic resonators that are directly integrated with circuits and enable a new generation of reconfigurable narrowband filters and oscillators. Research efforts related to the deposition of doped AlN films and the scaling of sputtered AlN films into the nano realm are also provided as examples of possible future material developments that could expand the range of applicability of AlN MEMS. C1 [Piazza, Gianluca] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Olsson, Roy H., III] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Ruby, Richard] Avago Technol, San Jose, CA USA. [Muralt, Paul] Swiss Fed Inst Technol, CH-1015 Lausanne, Switzerland. [Felmetsger, Valeriy] OEM Grp, Gilbert, AZ 85233 USA. RP Piazza, G (reprint author), Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. EM piazza@ece.cmu.edu; valeriy.felmetsger@oemgroupinc.com; paul.muralt@epfl.ch; rholsso@sandia.gov; rich.ruby@avagotech.com RI Muralt, Paul/C-5351-2008 OI Muralt, Paul/0000-0001-6004-1208 FU US Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors would like to thank all the students and postdoctoral researchers that work in Piazza's laboratory and the researchers of the Sandia microresonator team. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the US Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 68 TC 47 Z9 48 U1 7 U2 76 PU CAMBRIDGE UNIV PRESS PI NEW YORK PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA SN 0883-7694 EI 1938-1425 J9 MRS BULL JI MRS Bull. PD NOV PY 2012 VL 37 IS 11 BP 1051 EP 1061 DI 10.1557/mrs.2012.268 PG 11 WC Materials Science, Multidisciplinary; Physics, Applied SC Materials Science; Physics GA 036SG UT WOS:000311050200017 ER PT J AU Crabtree, GW Sarrao, JL AF Crabtree, G. W. Sarrao, J. L. TI Opportunities for mesoscale science SO MRS BULLETIN LA English DT Article ID BATTERIES; SYSTEMS AB The regime of mesoscale science, where the granularity of atoms and quantization of energy gives way to apparently continuous and infinitely divisible matter and energy, yields strikingly complex architectures, phenomena, and functionalities that control macroscopic material behavior. Research in mesoscale materials and chemical science is an opportunity space for next-generation discovery, science, technology, and innovation, with promise of new solutions for societal problems such as energy, environment, climate, advanced manufacturing, and economic growth. C1 [Crabtree, G. W.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Sarrao, J. L.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Crabtree, GW (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM crabtree@anl.gov; sarrao@lanl.gov FU Division of Materials Science and Engineering, Office of Basic Energy Sciences FX We thank our colleagues on the Mesoscale Science Subcommittee of the US DOE Basic Energy Sciences Advisory Committee and acknowledge the many individuals who provided input at www.meso2012.com. This work was supported in part by the Division of Materials Science and Engineering, Office of Basic Energy Sciences. NR 46 TC 30 Z9 30 U1 1 U2 59 PU CAMBRIDGE UNIV PRESS PI NEW YORK PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA SN 0883-7694 EI 1938-1425 J9 MRS BULL JI MRS Bull. PD NOV PY 2012 VL 37 IS 11 BP 1079 EP 1088 DI 10.1557/mrs.2012.274 PG 10 WC Materials Science, Multidisciplinary; Physics, Applied SC Materials Science; Physics GA 036SG UT WOS:000311050200020 ER PT J AU O'Hara, J Higgins, J D'Agostino, A AF O'Hara, John Higgins, James D'Agostino, Amy TI One person, x reactors SO NUCLEAR ENGINEERING INTERNATIONAL LA English DT Article C1 [O'Hara, John; Higgins, James] Brookhaven Natl Lab, New York, NY 11779 USA. [D'Agostino, Amy] US Nucl Regulatory Commiss, Washington, DC 20555 USA. RP O'Hara, J (reprint author), Brookhaven Natl Lab, New York, NY 11779 USA. EM ohara@bnl.gov RI Higgins, James/D-6822-2013 NR 0 TC 0 Z9 0 U1 0 U2 0 PU WILMINGTON PUBL PI SIDCUP PA WILMINGTON HOUSE, MAIDSTONE RD, FOOTS CRAY, SIDCUP DA14 SHZ, KENT, ENGLAND SN 0029-5507 J9 NUCL ENG INT JI Nucl. Eng. Int. PD NOV PY 2012 VL 57 IS 700 BP 31 EP 34 PG 4 WC Nuclear Science & Technology SC Nuclear Science & Technology GA 038OC UT WOS:000311183000010 ER PT J AU Alexandrov, BS Fukuyo, Y Lange, M Horikoshi, N Gelev, V Rasmussen, KO Bishop, AR Usheva, A AF Alexandrov, Boian S. Fukuyo, Yayoi Lange, Martin Horikoshi, Nobuo Gelev, Vladimir Rasmussen, Kim O. Bishop, Alan R. Usheva, Anny TI DNA breathing dynamics distinguish binding from nonbinding consensus sites for transcription factor YY1 in cells SO NUCLEIC ACIDS RESEARCH LA English DT Article ID BASAL TRANSCRIPTION; NONLINEAR MODEL; DENATURATION; INITIATION AB The genome-wide mapping of the major gene expression regulators, the transcription factors (TFs) and their DNA binding sites, is of great importance for describing cellular behavior and phenotypic diversity. Presently, the methods for prediction of genomic TF binding produce a large number of false positives, most likely due to insufficient description of the physiochemical mechanisms of protein-DNA binding. Growing evidence suggests that, in the cell, the double-stranded DNA (dsDNA) is subject to local transient strands separations (breathing) that contribute to genomic functions. By using site-specific chromatin immunopecipitations, gel shifts, BIOBASE data, and our model that accurately describes the melting behavior and breathing dynamics of dsDNA we report a specific DNA breathing profile found at YY1 binding sites in cells. We find that the genomic flanking sequence variations and SNPs, may exert long-range effects on DNA dynamics and predetermine YY1 binding. The ubiquitous TF YY1 has a fundamental role in essential biological processes by activating, initiating or repressing transcription depending upon the sequence context it binds. We anticipate that consensus binding sequences together with the related DNA dynamics profile may significantly improve the accuracy of genomic TF binding sites and TF binding-related functional SNPs. C1 [Alexandrov, Boian S.; Fukuyo, Yayoi; Lange, Martin; Horikoshi, Nobuo; Gelev, Vladimir; Usheva, Anny] Harvard Univ, Sch Med, Dept Med, Beth Israel Deaconess Med Ctr, Boston, MA 02215 USA. [Alexandrov, Boian S.; Rasmussen, Kim O.; Bishop, Alan R.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Horikoshi, Nobuo] Univ Texas SW Med Sch, Dept Radiat Oncol, Dallas, TX 75390 USA. RP Usheva, A (reprint author), Harvard Univ, Sch Med, Dept Med, Beth Israel Deaconess Med Ctr, Boston, MA 02215 USA. EM ausheva@bidmc.harvard.edu RI Rasmussen, Kim/B-5464-2009; Alexandrov, Boian/D-2488-2010 OI Rasmussen, Kim/0000-0002-4029-4723; Alexandrov, Boian/0000-0001-8636-4603 FU DOE [LANL] [LDRD 20110516ECR]; National Institutes of Health [ARRA supplement] [GM073911-04S]; National Nuclear Security Administration of the US Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396]; William F. Milton Award FX Funding for open access charge: DOE [LANL, LDRD 20110516ECR to B. A.]; National Institutes of Health [ARRA supplement GM073911-04S to A. U.]; contract from the National Nuclear Security Administration of the US Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396]; William F. Milton Award (to A.U.). NR 28 TC 16 Z9 16 U1 0 U2 6 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0305-1048 J9 NUCLEIC ACIDS RES JI Nucleic Acids Res. PD NOV PY 2012 VL 40 IS 20 BP 10116 EP 10123 DI 10.1093/nar/gks758 PG 8 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA 035TC UT WOS:000310970700022 PM 22904068 ER PT J AU Shiltsev, V AF Shiltsev, Vladimir TI Did Lomonosov see the Venusian atmosphere? replies SO PHYSICS TODAY LA English DT Editorial Material C1 Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. RP Shiltsev, V (reprint author), Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. EM shiltsev@fnal.gov NR 1 TC 0 Z9 0 U1 0 U2 0 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0031-9228 J9 PHYS TODAY JI Phys. Today PD NOV PY 2012 VL 65 IS 11 BP 12 EP 12 PG 1 WC Physics, Multidisciplinary SC Physics GA 037UG UT WOS:000311131400008 ER PT J AU Thompson, DJ Digel, SW Racusin, JL AF Thompson, David J. Digel, Seth W. Racusin, Judith L. TI Exploring the extreme universe with the Fermi Gamma-Ray Space Telescope SO PHYSICS TODAY LA English DT Article ID LARGE-AREA TELESCOPE C1 [Thompson, David J.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Digel, Seth W.] SLAC, Menlo Pk, CA USA. RP Thompson, DJ (reprint author), NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. RI Racusin, Judith/D-2935-2012 NR 9 TC 0 Z9 0 U1 0 U2 1 PU AMER INST PHYSICS PI MELVILLE PA CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA SN 0031-9228 J9 PHYS TODAY JI Phys. Today PD NOV PY 2012 VL 65 IS 11 BP 39 EP 45 PG 7 WC Physics, Multidisciplinary SC Physics GA 037UG UT WOS:000311131400020 ER PT J AU Crease, RP AF Crease, Robert P. TI Critical Point Primate physics SO PHYSICS WORLD LA English DT Editorial Material C1 [Crease, Robert P.] SUNY Stony Brook, Dept Philosophy, Stony Brook, NY 11790 USA. [Crease, Robert P.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Crease, RP (reprint author), SUNY Stony Brook, Dept Philosophy, Stony Brook, NY 11790 USA. EM rcrease@notes.cc.sunysb.edu NR 0 TC 0 Z9 0 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8585 J9 PHYS WORLD JI Phys. World PD NOV PY 2012 VL 25 IS 11 BP 18 EP 18 PG 1 WC Physics, Multidisciplinary SC Physics GA 036DS UT WOS:000311007200021 ER PT J AU Sweeney, LM Okolica, MR Gut, CP Gargas, ML AF Sweeney, Lisa M. Okolica, Michelle R. Gut, Chester P., Jr. Gargas, Michael L. TI Cancer mode of action, weight of evidence, and proposed cancer reference value for hexahydro-1,3,5-trinitro-1,3,5-triazine (RDX) SO REGULATORY TOXICOLOGY AND PHARMACOLOGY LA English DT Article DE RDX; Cancer; Mode of action; Hepatocellular carcinoma; Physiologically based pharmacokinetic (PBPK) modeling ID MICE PEROMYSCUS-MANICULATUS; 2,4,6-TRINITROTOLUENE TNT; SALMONELLA-TYPHIMURIUM; MUTAGENIC ACTIVITY; MAMMALIAN-CELLS; MUTATION ASSAY; METABOLITES; EXPOSURE; MOUSE; LIVER AB Hexahydro-1,3,5-trinitro-1,3,5-triazine (RDX, CAS No. 121-82-4) is a component of munitions formulations, and has been detected in groundwater samples collected at various US military sites. Clean up target levels for RDX may be derived based on consideration of acceptable cumulative human exposure as expressed in toxicity reference values. Evaluations of the cancer weight of evidence and possible modes of action (MOA) for RDX-induced cancer were conducted. It was concluded that the available data provide suggestive evidence of human carcinogenic potential for RDX. While a mutagenic/genotoxic MOA for RDX is unlikely, no alterative MOA is strongly supported by the available data. A nonlinear (threshold) approach to the assessment of human cancer risk was recommended, and a recommended chronic cancer reference dose of 0.08 mg/kg/day was derived. For comparison only, computations using a linear approach were also conducted, yielding a cancer risk specific dose of 0.000235 mg/kg/day for 1 in 105 risk; this value is 2.6-fold higher the current US EPA risk specific dose for 1 in 10(5) risk. Thus, cleanup standards based on human health risk from RDX exposure could potentially depend on the willingness of risk managers to accept a nonlinear MOA and nonlinear toxicity risk value derivation. Published by Elsevier Inc. C1 [Sweeney, Lisa M.] Henry M Jackson Fdn Adv Mil Med, Naval Med Res Unit Dayton, Wright Patterson AFB, OH 45433 USA. [Gut, Chester P., Jr.] Oak Ridge Inst Sci & Educ, Oak Ridge, TN USA. RP Sweeney, LM (reprint author), Henry M Jackson Fdn Adv Mil Med, Naval Med Res Unit Dayton, 2624 Q St,Bldg 851,Area B, Wright Patterson AFB, OH 45433 USA. EM lmsweeney@aol.com RI Sweeney, Lisa/K-5114-2012 OI Sweeney, Lisa/0000-0002-4672-7358 FU US Army Environmental Command, Installation and Restoration Program [61063] FX This work was sponsored by the US Army Environmental Command, Installation and Restoration Program, under Work Unit Number 61063. The sponsor's representatives, Drs. Mark Johnson, Desmond Bannon, Larry Williams, and Gunda Reddy, provided comments on a draft version of the manuscript and participated in the decision to submit the paper for publication. We thank Elizabeth Phillips, Tracy Doyle, and Mary Eaton from the Naval Medical Research Unit-Dayton for their contributions to the sample and data analysis. NR 68 TC 5 Z9 5 U1 3 U2 19 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0273-2300 J9 REGUL TOXICOL PHARM JI Regul. Toxicol. Pharmacol. PD NOV PY 2012 VL 64 IS 2 BP 205 EP 224 DI 10.1016/j.yrtph.2012.07.005 PG 20 WC Medicine, Legal; Pharmacology & Pharmacy; Toxicology SC Legal Medicine; Pharmacology & Pharmacy; Toxicology GA 036VX UT WOS:000311061500003 PM 22841928 ER PT J AU Sun, YG Liu, YZ Truong, TT Ren, Y AF Sun YuGang Liu YuZi Truong, Tu T. Ren Yang TI Thermal transformation of delta-MnO2 nanoflowers studied by in-situ TEM SO SCIENCE CHINA-CHEMISTRY LA English DT Article DE delta-MnO2 nanoflowers; alpha-MnO2; thermal annealing; in-situ TEM; mechanism study ID ELECTROCHEMICAL SUPERCAPACITORS; CAPACITANCE PROPERTIES; LITHIUM BATTERIES; MNO2; ELECTRODE AB In-situ transmission electron microscopy in combination with a heating stage has been employed to real-time monitor variations of delta-phase MnO2 nanoflowers in terms of their morphology and crystalline structures upon thermal annealing at elevated temperatures up to similar to 665 A degrees C. High-temperature annealing drives the diffusion of the small delta-MnO2 nanocrystallites within short distances less than 15 nm and the fusion of the adjacent delta-MnO2 nanocrystallites, leading to the formation of larger crystalline domains including highly crystalline nanorods. The annealed nanoflowers remain their overall flower-like morphology while they are converted to alpha-MnO2. The preferred transformation of the delta-MnO2 to the alpha-MnO2 can be ascribed to the close lattice spacing of most crystalline lattices between delta-MnO2 and alpha-MnO2, that might lead to a possible epitaxial growth of alpha-MnO2 lattices on the delta-MnO2 lattices during the thermal annealing process. C1 [Sun YuGang; Liu YuZi; Truong, Tu T.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Ren Yang] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. RP Sun, YG (reprint author), Argonne Natl Lab, Ctr Nanoscale Mat, 9700 S Cass Ave, Argonne, IL 60439 USA. EM ygsun@anl.gov RI Sun, Yugang /A-3683-2010; Truong, Tu/E-7029-2011; Liu, Yuzi/C-6849-2011 OI Sun, Yugang /0000-0001-6351-6977; FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work was performed at the Center for Nanoscale Materials, a U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility under contract No. DE-AC02-06CH11357. Use of the Electron Microscopy Center for Materials Research and Advanced Photon Source (Beam line 11-ID-C) at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under contract No. DE-AC02-06CH11357. NR 15 TC 3 Z9 3 U1 4 U2 64 PU SCIENCE PRESS PI BEIJING PA 16 DONGHUANGCHENGGEN NORTH ST, BEIJING 100717, PEOPLES R CHINA SN 1674-7291 J9 SCI CHINA CHEM JI Sci. China-Chem. PD NOV PY 2012 VL 55 IS 11 BP 2346 EP 2352 DI 10.1007/s11426-012-4688-5 PG 7 WC Chemistry, Multidisciplinary SC Chemistry GA 040DP UT WOS:000311301300011 ER PT J AU Burgess, D Mobius, E Scholer, M AF Burgess, D. Moebius, E. Scholer, M. TI Ion Acceleration at the Earth's Bow Shock SO SPACE SCIENCE REVIEWS LA English DT Review DE Ion acceleration; Bow shock; Space plasma; Collisionless shock; Particle acceleration ID FIELD-ALIGNED BEAMS; QUASI-PERPENDICULAR SHOCKS; HYDROMAGNETIC WAVE EXCITATION; MULTI-SPACECRAFT OBSERVATIONS; UPSTREAM PARTICLE EVENTS; SUPERCRITICAL COLLISIONLESS SHOCKS; INTERPLANETARY TRAVELING SHOCKS; PARALLEL SHOCKS; DIFFUSE IONS; SOLAR-WIND AB The Earth's bow shock is the most studied example of a collisionless shock in the solar system. It is also widely used to model or predict the behaviour at other astrophysical shock systems. Spacecraft observations, theoretical modelling and numerical simulations have led to a detailed understanding of the bow shock structure, the spatial organization of the components making up the shock interaction system, as well as fundamental shock processes such as particle heating and acceleration. In this paper we review the observations of accelerated ions at and upstream of the terrestrial bow shock and discuss the models and theories used to explain them. We describe the global morphology of the quasi-perpendicular and quasi-parallel shock regions and the foreshock. The acceleration processes for field-aligned beams and diffuse ion distribution types are discussed with connection to foreshock morphology and shock structure. The different possible mechanisms for extracting solar wind ions into the acceleration processes are also described. Despite several decades of study, there still remain some unsolved problems concerning ion acceleration at the bow shock, and we summarize these challenges. C1 [Burgess, D.] Queen Mary Univ London, Astron Unit, London E1 4NS, England. [Moebius, E.] Univ New Hampshire, Ctr Space Sci, Durham, NH 03824 USA. [Moebius, E.] Univ New Hampshire, Dept Phys, Durham, NH 03824 USA. [Moebius, E.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Scholer, M.] Max Planck Inst Extraterr Phys, D-85740 Garching, Germany. RP Burgess, D (reprint author), Queen Mary Univ London, Astron Unit, London E1 4NS, England. EM D.Burgess@qmul.ac.uk OI Moebius, Eberhard/0000-0002-2745-6978 FU STFC [ST/H002731/1]; NASA [NNX11AB65G]; U.S. Department of Energy through LANL's Laboratory Directed Research and Development (LDRD) Program; Institute Geophysics and Planetary Physics FX The authors thank ISSI for support to attend the workshop "Particle Acceleration in Cosmic Plasmas." D. Burgess acknowledges support of STFC grant ST/H002731/1. E. Mobius acknowledges support of NASA grant NNX11AB65G, and gratefully acknowledges the support of the U.S. Department of Energy through LANL's Laboratory Directed Research and Development (LDRD) Program and Institute Geophysics and Planetary Physics. NR 119 TC 24 Z9 24 U1 1 U2 11 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0038-6308 EI 1572-9672 J9 SPACE SCI REV JI Space Sci. Rev. PD NOV PY 2012 VL 173 IS 1-4 BP 5 EP 47 DI 10.1007/s11214-012-9901-5 PG 43 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 034MR UT WOS:000310878100002 ER PT J AU Birn, J Artemyev, AV Baker, DN Echim, M Hoshino, M Zelenyi, LM AF Birn, J. Artemyev, A. V. Baker, D. N. Echim, M. Hoshino, M. Zelenyi, L. M. TI Particle Acceleration in the Magnetotail and Aurora SO SPACE SCIENCE REVIEWS LA English DT Review DE Magnetotail; Aurora; Reconnection; Substorm injections ID PARALLEL ELECTRIC-FIELDS; PLASMA SHEET BOUNDARY; COLLISIONLESS MAGNETIC RECONNECTION; CURRENT-VOLTAGE RELATIONSHIP; DRIFT-KINK INSTABILITY; SPACE-CHARGE CONTROL; MODEL CURRENT SHEETS; THIN CURRENT SHEETS; SCALE ALFVEN WAVES; DOUBLE-LAYERS AB This paper deals with acceleration processes in the magnetotail and the processes that enhance particle precipitation from the tail into the ionosphere through electric fields in the auroral acceleration region, generating or intensifying discrete auroral arcs. Particle acceleration in the magnetotail is closely related to substorms and the occurrence, and consequences, of magnetic reconnection. We discuss major advances in the understanding of relevant acceleration processes on the basis of simple analytical models, magnetohydrodynamic and test particle simulations, as well as full electromagnetic particle-in-cell simulations. The auroral acceleration mechanisms are not fully understood, although several, sometimes competing, theories and models received experimental support during the last decades. We review recent advances that emphasize the role of parallel electric fields produced by quasi-stationary or Alfvenic processes. C1 [Birn, J.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Birn, J.] Space Sci Inst, Boulder, CO 80301 USA. [Artemyev, A. V.; Zelenyi, L. M.] Russian Acad Sci, Space Res Inst, Moscow, Russia. [Baker, D. N.] U Colorado, Lab Atmospher & Space Phys, Boulder, CO USA. [Echim, M.] Belgian Inst Space Aeron, Brussels, Belgium. [Echim, M.] Inst Space Sci, Bucharest, Romania. [Hoshino, M.] Univ Tokyo, Space & Planetary Sci Grp, Tokyo, Japan. RP Birn, J (reprint author), Los Alamos Natl Lab, POB 1663,MS 466, Los Alamos, NM 87545 USA. EM jbirn@lanl.gov; Ante0226@yandex.ru; Daniel.baker@lasp.colorado.edu; marius.echim@oma.be; hoshino@eps.s.u-tokyo.ac.jp; iki@cosmos.ru RI Echim, Marius/F-1813-2010 OI Echim, Marius/0000-0001-7038-9494 FU RFBR [10-02-93114, NIII-3200.2010.2]; NASA SRT; NASA MMS; Belgian Office for Science (Belspo) [MO/35/031]; European Space Agency, PECS contract [98049/2007]; International Space Science Institute (ISSI) FX The work of A.A. and L.Z. was supported by RFBR (No. 10-02-93114), grants of Leading Schools NIII-3200.2010.2. J.B. acknowledges support by NASA SR&T and MMS grants. M. E. acknowledges support from the Belgian Office for Science (Belspo), grant MO/35/031 and from the European Space Agency, PECS contract 98049/2007(KEEV). The authors thank the International Space Science Institute (ISSI) and the organizing committee for support and the opportunity to participate in the ISSI Workshop on Particle Acceleration in Cosmic Plasmas. NR 252 TC 70 Z9 70 U1 3 U2 47 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0038-6308 EI 1572-9672 J9 SPACE SCI REV JI Space Sci. Rev. PD NOV PY 2012 VL 173 IS 1-4 BP 49 EP 102 DI 10.1007/s11214-012-9874-4 PG 54 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 034MR UT WOS:000310878100003 ER PT J AU Lazarian, A Vlahos, L Kowal, G Yan, H Beresnyak, A Dal Pino, EMD AF Lazarian, A. Vlahos, L. Kowal, G. Yan, H. Beresnyak, A. de Gouveia Dal Pino, E. M. TI Turbulence, Magnetic Reconnection in Turbulent Fluids and Energetic Particle Acceleration SO SPACE SCIENCE REVIEWS LA English DT Review DE Turbulence; Magnetic reconnection; Acceleration; Cosmic rays ID GAMMA-RAY BURSTS; COMPRESSIBLE MAGNETOHYDRODYNAMIC TURBULENCE; ANOMALOUS COSMIC-RAYS; PITCH-ANGLE SCATTERING; DIFFUSIVE SHOCK ACCELERATION; FOKKER-PLANCK COEFFICIENT; SOLAR-WIND TERMINATION; SCALE ATOMIC-STRUCTURE; ALFVEN WAVE-PACKETS; INTERSTELLAR-MEDIUM AB Turbulence is ubiquitous in astrophysics. It radically changes many astrophysical phenomena, in particular, the propagation and acceleration of cosmic rays. We present the modern understanding of compressible magnetohydrodynamic (MHD) turbulence, in particular its decomposition into Alfv,n, slow and fast modes, discuss the density structure of turbulent subsonic and supersonic media, as well as other relevant regimes of astrophysical turbulence. All this information is essential for understanding the energetic particle acceleration that we discuss further in the review. For instance, we show how fast and slow modes accelerate energetic particles through the second order Fermi acceleration, while density fluctuations generate magnetic fields in pre-shock regions enabling the first order Fermi acceleration of high energy cosmic rays. Very importantly, however, the first order Fermi cosmic ray acceleration is also possible in sites of magnetic reconnection. In the presence of turbulence this reconnection gets fast and we present numerical evidence supporting the predictions of the Lazarian and Vishniac (Astrophys. J. 517:700-718, 1999) model of fast reconnection. The efficiency of this process suggests that magnetic reconnection can release substantial amounts of energy in short periods of time. As the particle tracing numerical simulations show that the particles can be efficiently accelerated during the reconnection, we argue that the process of magnetic reconnection may be much more important for particle acceleration than it is currently accepted. In particular, we discuss the acceleration arising from reconnection as a possible origin of the anomalous cosmic rays measured by Voyagers as well as the origin cosmic ray excess in the direction of Heliotail. C1 [Lazarian, A.] Univ Wisconsin, Dept Astron, Madison, WI 53706 USA. [Vlahos, L.] Univ Thessaloniki, Dept Phys, Thessaloniki 54124, Greece. [Kowal, G.; de Gouveia Dal Pino, E. M.] Univ Sao Paulo, Inst Astron Geofis & Ciencias Atmosfer, BR-05508090 Sao Paulo, Brazil. [Yan, H.] Peking Univ, Kavli Inst, Beijing 100871, Peoples R China. [Beresnyak, A.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Beresnyak, A.] Ruhr Univ Bochum, D-44789 Bochum, Germany. RP Lazarian, A (reprint author), Univ Wisconsin, Dept Astron, 475 N Charter St, Madison, WI 53706 USA. EM lazarian@astro.wisc.edu; vlahos@astro.auth.gr; kowal@astro.iag.usp.br; hryan@pku.edu.cn; beresnyak@wisc.edu; dalpino@astro.iag.usp.br RI Kowal, Grzegorz/K-5667-2012; 7, INCT/H-6207-2013; Astrofisica, Inct/H-9455-2013; de Gouveia Dal Pino, Elisabete/H-9560-2013; OI Kowal, Grzegorz/0000-0002-0176-9909; de Gouveia Dal Pino, Elisabete/0000-0001-8058-4752; Beresnyak, Andrey/0000-0002-2124-7024 FU NASA [NNX09AH78G]; NSF Center for Magnetic Self-Organization; FAPESP (Brazil) [2009/50053-8, 2006/50654-3]; CNPq (Brazil) [300083/94-7] FX A. Lazarian's research is supported by the NASA Grant NNX09AH78G, as well as the support of the NSF Center for Magnetic Self-Organization. The Humboldt Award at the Universities of Cologne and Bochum, as well as Vilas Associate Award and the hospitality of the International Institute of Physics (Brazil) are acknowledged. G. Kowal's research is supported by FAPESP (Brazil) grant No. 2009/50053-8. E. de Gouveia Dal Pino also acknowledges partial supported from FAPESP (Brazil: grant No. 2006/50654-3) and from CNPq (Brazil; grant No. 300083/94-7). We thank the anonymous referee for comments and suggestions that improved the paper. HY acknowledges the Visiting Professorship from IIP. NR 277 TC 37 Z9 38 U1 3 U2 12 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0038-6308 EI 1572-9672 J9 SPACE SCI REV JI Space Sci. Rev. PD NOV PY 2012 VL 173 IS 1-4 BP 557 EP 622 DI 10.1007/s11214-012-9936-7 PG 66 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 034MR UT WOS:000310878100018 ER PT J AU Kiener, D Kaufmann, P Minor, AM AF Kiener, Daniel Kaufmann, Petra Minor, Andrew M. TI Strength, Hardening, and Failure Observed by In Situ TEM Tensile Testing SO ADVANCED ENGINEERING MATERIALS LA English DT Article ID DISLOCATION NUCLEATION; CRYSTAL PLASTICITY; METALLIC-GLASS; SINGLE-CRYSTAL; SIZE; DEFORMATION; COPPER; COMPRESSION; MICROPILLARS; NANOPILLARS AB We present in situ transmission electron microscope tensile tests on focused ion beam fabricated single and multiple slip oriented Cu tensile samples with thicknesses in the range of 100-200 nm. Both crystal orientations fail by localized shear. While failure occurs after a few percent plastic strain and limited hardening in the single slip case, the multiple slip samples exhibit extended homogenous deformation and necking due to the activation of multiple dislocation sources in conjunction with significant hardening. The hardening behavior at 1% plastic strain is even more pronounced compared to compression samples of the same orientation due to the absence of sample taper and the interface to the compression platen. Moreover, we show for the first time that the strain rate sensitivity of such FIB prepared samples is an order of magnitude higher than that of bulk Cu. C1 [Kiener, Daniel; Kaufmann, Petra] Univ Leoben, Dept Mat Phys, A-8700 Leoben, Austria. [Kiener, Daniel; Minor, Andrew M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Natl Ctr Elect Microscopy, Berkeley, CA 94720 USA. [Minor, Andrew M.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. RP Kiener, D (reprint author), Univ Leoben, Dept Mat Phys, Jahnstr 12, A-8700 Leoben, Austria. EM daniel.kiener@unileoben.ac.at RI Kiener, Daniel/B-2202-2008 OI Kiener, Daniel/0000-0003-3715-3986 FU National Center for Electron Microscopy, Lawrence Berkeley National Laboratory; U.S. Department of Energy [DE-AC02-05CH11231]; Austrian Science Fund (FWF) [J2834-N20] FX This work was supported by the National Center for Electron Microscopy, Lawrence Berkeley National Laboratory, which is funded by the U.S. Department of Energy under Contract # DE-AC02-05CH11231. DK gratefully acknowledges financial support of the Austrian Science Fund (FWF) through the project J2834-N20. Supporting Information is available online from Wiley Online Library or from the author. NR 62 TC 8 Z9 8 U1 5 U2 73 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA BOSCHSTRASSE 12, D-69469 WEINHEIM, GERMANY SN 1438-1656 J9 ADV ENG MATER JI Adv. Eng. Mater. PD NOV PY 2012 VL 14 IS 11 SI SI BP 960 EP 967 DI 10.1002/adem.201200031 PG 8 WC Materials Science, Multidisciplinary SC Materials Science GA 030WG UT WOS:000310600200007 ER PT J AU Broering, TM Lian, YS Henshaw, W AF Broering, Timothy M. Lian, Yongsheng Henshaw, William TI Numerical Investigation of Energy Extraction in a Tandem Flapping Wing Configuration SO AIAA JOURNAL LA English DT Article ID DRAGONFLY FLIGHT; AERODYNAMIC FORCES; POWER REQUIREMENTS; HIGH-SPEED; FLOW; AIRFOILS; SIMULATION; EFFICIENCY AB A number of flying insects make use of tandem-wing configurations, suggesting that such a setup may have potential advantages over a single wing at low Reynolds numbers. Dragonflies, which are fast and highly maneuverable, demonstrate well the potential performance of such a design. In this paper, a tandem-wing flapping configuration is simulated at a Reynolds number of 10,000 using an incompressible Navier-Stokes solver and an overlapping grid method. The flapping motion consists of a simple sinusoidal pitch and plunge motion with a spacing of one chord length between both wings. The arrangement was tested at a Strouhal number of 0.3 for three different phase angles: 0, 90, and 180 deg. The aerodynamics of the hindwing was compared in detail to a single wing, with the same geometry and undergoing the same flapping kinematics, to determine the effect of vortex shedding from the forewing on the hindwing, as well as how the phase angle affects the interaction. The average lift, thrust, and power coefficients and the average efficiency of the fore- and hindwings were compared with a single wing to determine how the tandem-wing interaction affects performance. The results show that adjusting the phase angle allows the tandem wing to change the flight mode. At 0 deg phase lag, the tandem wing produces high thrust at high propulsive efficiency, but low lift efficiency. Switching to 90/180 deg phase lag decreases the thrust production and propulsive efficiency but greatly increases the lift efficiency. At 90/180 deg, the power coefficient is much lower than at 0 deg, due to the hindwing extracting energy from the wake of the forewing. C1 [Broering, Timothy M.; Lian, Yongsheng] Univ Louisville, Dept Mech Engn, Louisville, KY 40292 USA. [Henshaw, William] Lawrence Livermore Natl Lab, Ctr Appl Sci Comp, Livermore, CA 94551 USA. RP Broering, TM (reprint author), Univ Louisville, Dept Mech Engn, Louisville, KY 40292 USA. FU U.S. Air Force; Intramural Research Incentive Grant from the Office of the Executive Vice President for Research of the University of Louisville FX This work is partially supported by U.S. Air Force and by an Intramural Research Incentive Grant from the Office of the Executive Vice President for Research of the University of Louisville. NR 39 TC 15 Z9 16 U1 1 U2 19 PU AMER INST AERONAUTICS ASTRONAUTICS PI RESTON PA 1801 ALEXANDER BELL DRIVE, STE 500, RESTON, VA 22091-4344 USA SN 0001-1452 EI 1533-385X J9 AIAA J JI AIAA J. PD NOV PY 2012 VL 50 IS 11 BP 2295 EP 2307 DI 10.2514/1.J051104 PG 13 WC Engineering, Aerospace SC Engineering GA 030GM UT WOS:000310559000002 ER PT J AU Ansari, N Pisciuneri, PH Strakey, PA Givi, P AF Ansari, N. Pisciuneri, P. H. Strakey, P. A. Givi, P. TI Scalar-Filtered Mass-Density-Function Simulation of Swirling Reacting Flows on Unstructured Grids SO AIAA JOURNAL LA English DT Article ID LARGE-EDDY SIMULATION; SANDIA FLAME-D; TURBULENT COMBUSTION; JET FLAMES; LES; FORMULATION; DIFFUSION; MODEL; EQUATIONS; TRANSPORT AB The scalar-filtered mass-density-function methodology is employed for large-eddy simulation of two swirl-stabilized nonpremixed flames. These are low-swirl (SM1) and high-swirl (SMA2) Sydney methane flames, both of which have been the subject of detailed laboratory measurements. Combustion chemistry is modeled via a flamelet model for the low-swirl flame, and a detailed finite-rate kinetics model for the high-swirl flame. The scalar-filtered mass-density-function is simulated by a Lagrangian Monte Carlo method on a domain discretized by unstructured grids. The simulated results are assessed via comparison with experimental data and show very good agreement. This demonstrates the capability of scalar-filtered mass-density-function for large-eddy simulation of complex flows and warrants future applications of the methodology for large-eddy simulation of practical combustor configurations. C1 [Ansari, N.; Pisciuneri, P. H.; Givi, P.] Univ Pittsburgh, Dept Mech Engn & Mat Sci, Pittsburgh, PA 15261 USA. [Ansari, N.] ANSYS Inc, Canonsburg, PA 15317 USA. [Strakey, P. A.] Natl Energy Technol Lab, Morgantown, WV 26507 USA. RP Ansari, N (reprint author), Univ Pittsburgh, Dept Mech Engn & Mat Sci, Pittsburgh, PA 15261 USA. FU U.S. Department of Energy [RES10000027/96]; National Center for Hypersonic Combined Cycle Propulsion under U.S. Air Force Office of Scientific Research (AFOSR) [FA-9550-09-1-0611]; National Science Foundation [OCI-1053575] FX This research was sponsored partly by the U.S. Department of Energy under contract RES10000027/96 and partly by the National Center for Hypersonic Combined Cycle Propulsion under U.S. Air Force Office of Scientific Research (AFOSR) grant FA-9550-09-1-0611. The technical monitors on this grant are Chiping Li (AFOSR), Aaron Auslender (NASA), and Rick Gaffney (NASA). Computational resources are partly provided by the Extreme Science and Engineering Discovery Environment, which is supported by the National Science Foundation under grant OCI-1053575. NR 55 TC 7 Z9 7 U1 1 U2 9 PU AMER INST AERONAUT ASTRONAUT PI RESTON PA 1801 ALEXANDER BELL DRIVE, STE 500, RESTON, VA 22091-4344 USA SN 0001-1452 J9 AIAA J JI AIAA J. PD NOV PY 2012 VL 50 IS 11 BP 2476 EP 2482 DI 10.2514/1.J051671 PG 7 WC Engineering, Aerospace SC Engineering GA 030GM UT WOS:000310559000015 ER PT J AU Beresh, SJ Henfling, JF Spillers, RW AF Beresh, Steven J. Henfling, John F. Spillers, Russell W. TI Turbulence of a Fin Trailing Vortex in Subsonic Compressible Flow SO AIAA JOURNAL LA English DT Article ID PARTICLE IMAGE VELOCIMETRY; WING-TIP VORTEX; NEAR-FIELD; VORTICES; WATER; ORIGIN; LAYER AB Stereoscopic Particle Image Velocimetry data of a trailing vortex shed from a tapered fin installed on a wind-tunnel wall have been analyzed to provide turbulent statistics. After correcting for the effects of vortex meander, the radial and azimuthal turbulent normal stresses are smallest at the vortex center, reaching a maximum around its periphery to produce an annulus of turbulence. Conversely, the streamwise turbulent stress peaks at the vortex center. The ringed turbulent structure is consistent with rotation stabilizing the flow in the vortex core, whereas a fluctuating axial velocity contributes to vortex decay. All three turbulent normal stresses decay with downstream distance. Turbulent shear stresses also decay with downstream distance but possess a relatively small magnitude, suggesting minimal coupling between turbulent velocity components. The vortex turbulence is strongly anisotropic in a manner that varies greatly with spatial position. As the vortex strength is reduced, the axial turbulent normal stress diminishes more sharply than the two cross-plane turbulent normal stresses, possibly because the latter components are influenced by external turbulence spiraling towards the vortex core. The turbulent shear stresses do not show discernable reductions in magnitude with lower vortex strength. C1 [Beresh, Steven J.; Henfling, John F.; Spillers, Russell W.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Beresh, SJ (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM sjberes@sandia.gov FU Sandia National Laboratories; United States Department of Energy; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported by Sandia National Laboratories and the United States Department of Energy. Sandia is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL85000. NR 41 TC 0 Z9 0 U1 1 U2 3 PU AMER INST AERONAUT ASTRONAUT PI RESTON PA 1801 ALEXANDER BELL DRIVE, STE 500, RESTON, VA 22091-4344 USA SN 0001-1452 J9 AIAA J JI AIAA J. PD NOV PY 2012 VL 50 IS 11 BP 2609 EP 2622 DI 10.2514/1.J051904 PG 14 WC Engineering, Aerospace SC Engineering GA 030GM UT WOS:000310559000027 ER PT J AU Karasavvas, N Billings, E Rao, M Williams, C Zolla-Pazner, S Bailer, RT Koup, RA Madnote, S Arworn, D Shen, XY Tomaras, GD Currier, JR Jiang, M Magaret, C Andrews, C Gottardo, R Gilbert, P Cardozo, TJ Rerks-Ngarm, S Nitayaphan, S Pitisuttithum, P Kaewkungwal, J Paris, R Greene, K Gao, HM Gurunathan, S Tartaglia, J Sinangil, F Korber, BT Montefiori, DC Mascola, JR Robb, ML Haynes, BF Ngauy, V Michael, NL Kim, JH de Souza, MS AF Karasavvas, Nicos Billings, Erik Rao, Mangala Williams, Constance Zolla-Pazner, Susan Bailer, Robert T. Koup, Richard A. Madnote, Sirinan Arworn, Duangnapa Shen, Xiaoying Tomaras, Georgia D. Currier, Jeffrey R. Jiang, Mike Magaret, Craig Andrews, Charla Gottardo, Raphael Gilbert, Peter Cardozo, Timothy J. Rerks-Ngarm, Supachai Nitayaphan, Sorachai Pitisuttithum, Punnee Kaewkungwal, Jaranit Paris, Robert Greene, Kelli Gao, Hongmei Gurunathan, Sanjay Tartaglia, Jim Sinangil, Faruk Korber, Bette T. Montefiori, David C. Mascola, John R. Robb, Merlin L. Haynes, Barton F. Ngauy, Viseth Michael, Nelson L. Kim, Jerome H. de Souza, Mark S. CA MOPH TAVEG Collaboration TI The Thai Phase III HIV Type 1 Vaccine Trial (RV144) Regimen Induces Antibodies That Target Conserved Regions Within the V2 Loop of gp120 SO AIDS RESEARCH AND HUMAN RETROVIRUSES LA English DT Article ID IMMUNODEFICIENCY-VIRUS TYPE-1; RECOMBINANT GLYCOPROTEIN-120 VACCINE; QUATERNARY NEUTRALIZING EPITOPE; HIV-1/SIV CHIMERIC VIRUS; ENVELOPE GLYCOPROTEIN; EFFICACY TRIAL; HETEROSEXUAL TRANSMISSION; INTEGRIN ALPHA(4)BETA(7); MONOCLONAL-ANTIBODIES; CANARYPOX VACCINE AB The Thai Phase III clinical trial (RV144) showed modest efficacy in preventing HIV-1 acquisition. Plasma collected from HIV-1-uninfected trial participants completing all injections with ALVAC-HIV (vCP1521) prime and AIDSVAX B/E boost were tested for antibody responses against HIV-1 gp120 envelope (Env). Peptide microarray analysis from six HIV-1 subtypes and group M consensus showed that vaccination induced antibody responses to the second variable (V2) loop of gp120 of multiple subtypes. We further evaluated V2 responses by ELISA and surface plasmon resonance using cyclic (Cyc) and linear V2 loop peptides. Thirty-one of 32 vaccine recipients tested (97%) had antibody responses against Cyc V2 at 2 weeks postimmunization with a reciprocal geometric mean titer (GMT) of 1100 (range: 200-3200). The frequency of detecting plasma V2 antibodies declined to 19% at 28 weeks post-last injection (GMT: 110, range: 100-200). Antibody responses targeted the mid-region of the V2 loop that contains conserved epitopes and has the amino acid sequence KQKVHALFYKLDIVPI (HXB2 Numbering sequence 169-184). Valine at position 172 was critical for antibody binding. The frequency of V3 responses at 2 weeks postimmunization was modest (18/32, 56%) with a GMT of 185 (range: 100-800). In contrast, naturally infected HIV-1 individuals had a lower frequency of antibody responses to V2 (10/20, 50%; p = 0.003) and a higher frequency of responses to V3 (19/20, 95%), with GMTs of 400 (range: 100-3200) and 3570 (range: 200-12,800), respectively. RV144 vaccination induced antibodies that targeted a region of the V2 loop that contains conserved epitopes. Early HIV-1 transmission events involve V2 loop interactions, raising the possibility that anti-V2 antibodies in RV144 may have contributed to viral inhibition. C1 [Karasavvas, Nicos; Madnote, Sirinan; Arworn, Duangnapa; Ngauy, Viseth; de Souza, Mark S.] Armed Forces Res Inst Med Sci, US Army Med Component, Dept Retrovirol, Bangkok 10400, Thailand. [Billings, Erik; Currier, Jeffrey R.; Andrews, Charla; Robb, Merlin L.] Henry M Jackson Fdn Adv Mil Med, US Mil HIV Res Program MHRP, Rockville, MD USA. [Rao, Mangala; Paris, Robert; Michael, Nelson L.; Kim, Jerome H.] Walter Reed Army Inst Res, USMHRP, Silver Spring, MD USA. [Williams, Constance; Zolla-Pazner, Susan; Cardozo, Timothy J.] NYU, Sch Med, Dept Pathol, New York, NY USA. [Williams, Constance; Zolla-Pazner, Susan; Cardozo, Timothy J.] NYU, Sch Med, Dept Pharmacol, New York, NY USA. [Zolla-Pazner, Susan] Vet Affairs Harbor Healthcare Syst, New York, NY USA. [Bailer, Robert T.; Koup, Richard A.] NIAID, Immunol Lab, Vaccine Res Ctr, NIH, Bethesda, MD 20892 USA. [Shen, Xiaoying; Tomaras, Georgia D.; Haynes, Barton F.] Duke Univ, Med Ctr, Duke Human Vaccine Inst, Durham, NC USA. [Jiang, Mike; Magaret, Craig; Gottardo, Raphael; Gilbert, Peter] Fred Hutchinson Canc Res Ctr, Vaccine & Infect Dis Div, Seattle, WA 98104 USA. [Rerks-Ngarm, Supachai] Minist Publ Hlth, Dept Dis Control, Nonthaburi, Thailand. [Nitayaphan, Sorachai] Armed Forces Res Inst Med Sci, Royal Thai Army Component, Bangkok 10400, Thailand. [Pitisuttithum, Punnee] Mahidol Univ, Fac Trop Med, Vaccine Trial Ctr, Bangkok, Thailand. [Pitisuttithum, Punnee] Mahidol Univ, Fac Trop Med, Dept Clin Trop Med, Bangkok, Thailand. [Kaewkungwal, Jaranit] Mahidol Univ, Fac Trop Med, Ctr Excellence Biomed & Publ Hlth Informat BIOPHI, Bangkok, Thailand. [Paris, Robert] Walter Reed Natl Mil Med Ctr, Bethesda, MD USA. [Greene, Kelli; Gao, Hongmei; Montefiori, David C.; Mascola, John R.] Duke Univ, Med Ctr, Dept Surg, Durham, NC 27710 USA. [Gurunathan, Sanjay; Tartaglia, Jim] Sanofi Pasteur, Swiftwater, PA USA. [Sinangil, Faruk] Global Solut Infect Dis, San Francisco, CA USA. [Korber, Bette T.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM USA. RP Karasavvas, N (reprint author), Armed Forces Res Inst Med Sci, US Army Med Component, Dept Retrovirol, 315-6 Rajvithi Rd, Bangkok 10400, Thailand. EM karasavvan@afrims.org RI Tomaras, Georgia/J-5041-2016; OI Korber, Bette/0000-0002-2026-5757 FU U.S. Army Medical Research and Materiel Command (USAMRMC) [Y1-AI-2642-12]; National Institutes of Allergy and Infectious Diseases; Henry M. Jackson Foundation for the Advancement of Military Medicine [W81XWH-07-2-0067]; U.S. Department of Defense [W81XWH-07-2-0067]; U.S. National Institute of Allergy and Infectious Diseases; Bill and Melinda Gates Foundation [OPP38744]; NIH Vaccine Research Center; NIH [HL59725, AI084119]; Department of Veterans Affairs; Bill and Melinda Gates Foundation Collaboration for AIDS Vaccine Discovery FX The authors thank SCHARP for assisting with the microarray analysis, James Swetnam for providing the biotinylated subtype B linear peptides, Kelly Soderberg for coordination of sample shipment and project management, Rob O'Connell for constructive reading of the manuscript, Robert Parks, Ryan Meyerhoff, and Krissey Lloyd for ELISA technical assistance, and Ellen Turk for performing the peptide microarray analysis. These studies were supported in part by an Interagency Agreement Y1-AI-2642-12 between U.S. Army Medical Research and Materiel Command (USAMRMC) and the National Institutes of Allergy and Infectious Diseases. In addition, this work was supported by a cooperative agreement (W81XWH-07-2-0067) between the Henry M. Jackson Foundation for the Advancement of Military Medicine and the U.S. Department of Defense. This research was funded, in part, by the U.S. National Institute of Allergy and Infectious Diseases. Peptide microarray work was funded by the Bill and Melinda Gates Foundation's Collaboration for AIDS Vaccine Discovery (OPP38744) and the NIH Vaccine Research Center. S.Z.P. and T.J.C. receive funding from NIH Grants HL59725 (S.Z.P.) and AI084119 (T.J.C.) and the Department of Veterans Affairs. Supported in part by grants from the Bill and Melinda Gates Foundation Collaboration for AIDS Vaccine Discovery to Dr. Haynes. NR 69 TC 82 Z9 82 U1 4 U2 16 PU MARY ANN LIEBERT INC PI NEW ROCHELLE PA 140 HUGUENOT STREET, 3RD FL, NEW ROCHELLE, NY 10801 USA SN 0889-2229 J9 AIDS RES HUM RETROV JI Aids Res. Hum. Retrovir. PD NOV PY 2012 VL 28 IS 11 BP 1444 EP 1457 DI 10.1089/aid.2012.0103 PG 14 WC Immunology; Infectious Diseases; Virology SC Immunology; Infectious Diseases; Virology GA 032XP UT WOS:000310754100009 PM 23035746 ER PT J AU Barth, S AF Barth, Susanne TI Breeding strategies for forage and grass improvement PREFACE SO ANNALS OF BOTANY LA English DT Editorial Material C1 TEAGASC, Crops Environm & Land Use Programme, Oak Pk Res Ctr, Carlow, Ireland. RP Barth, S (reprint author), TEAGASC, Crops Environm & Land Use Programme, Oak Pk Res Ctr, Carlow, Ireland. EM Susanne.Barth@teagasc.ie RI Barth, Susanne/P-3366-2014 OI Barth, Susanne/0000-0002-4104-5964 NR 8 TC 3 Z9 3 U1 0 U2 13 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0305-7364 J9 ANN BOT-LONDON JI Ann. Bot. PD NOV PY 2012 VL 110 IS 6 BP 1261 EP 1262 DI 10.1093/aob/mcs219 PG 2 WC Plant Sciences SC Plant Sciences GA 027RV UT WOS:000310371800016 PM 23091094 ER PT J AU Diekmann, K Hodkinson, TR Barth, S AF Diekmann, Kerstin Hodkinson, Trevor R. Barth, Susanne TI New chloroplast microsatellite markers suitable for assessing genetic diversity of Lolium perenne and other related grass species SO ANNALS OF BOTANY LA English DT Article DE Lolium perenne; perennial ryegrass; Poaceae; chloroplast microsatellite markers; chloroplast genome; genetic diversity ID DNA-SEQUENCES; INTEGRATED SOFTWARE; MOLECULAR DIVERSITY; POPULATION-GENETICS; UNIVERSAL PRIMERS; ORGANELLE DNA; RYEGRASS; POACEAE; NUCLEAR; GENOME AB Lolium perenne (perennial ryegrass) is the most important forage grass species of temperate regions. We have previously released the chloroplast genome sequence of L. perenne oCashel'. Here nine chloroplast microsatellite markers are published, which were designed based on knowledge about genetically variable regions within the L. perenne chloroplast genome. These markers were successfully used for characterizing the genetic diversity in Lolium and different grass species. Chloroplast genomes of 14 Poaceae taxa were screened for mononucleotide microsatellite repeat regions and primers designed for their amplification from nine loci. The potential of these markers to assess genetic diversity was evaluated on a set of 16 Irish and 15 European L. perenne ecotypes, nine L. perenne cultivars, other Lolium taxa and other grass species. All analysed Poaceae chloroplast genomes contained more than 200 mononucleotide repeats (chloroplast simple sequence repeats, cpSSRs) of at least 7 bp in length, concentrated mainly in the large single copy region of the genome. Nucleotide composition varied considerably among subfamilies (with Pooideae biased towards poly A repeats). The nine new markers distinguish L. perenne from all non-Lolium taxa. TeaCpSSR28 was able to distinguish between all Lolium species and Lolium multiflorum due to an elongation of an A(8) mononucleotide repeat in L. multiflorum. TeaCpSSR31 detected a considerable degree of microsatellite length variation and single nucleotide polymorphism. TeaCpSSR27 revealed variation within some L. perenne accessions due to a 44-bp indel and was hence readily detected by simple agarose gel electrophoresis. Smaller insertion/deletion events or single nucleotide polymorphisms detected by these new markers could be visualized by polyacrylamide gel electrophoresis or DNA sequencing, respectively. The new markers are a valuable tool for plant breeding companies, seed testing agencies and the wider scientific community due to their ability to monitor genetic diversity within breeding pools, to trace maternal inheritance and to distinguish closely related species. C1 [Diekmann, Kerstin; Barth, Susanne] Oak Pk Res Ctr, Teagasc Crops Environm & Land Use Programme, Carlow, Ireland. [Diekmann, Kerstin; Hodkinson, Trevor R.] Trinity Coll Dublin, Sch Nat Sci, Dublin 2, Ireland. [Hodkinson, Trevor R.] Trinity Coll Dublin, Trinity Ctr Biodivers Res, Dublin 2, Ireland. RP Diekmann, K (reprint author), Oak Pk Res Ctr, Teagasc Crops Environm & Land Use Programme, Carlow, Ireland. EM kerstin.diekmann@gmail.com RI Hodkinson, Trevor/F-6850-2014; Barth, Susanne/P-3366-2014 OI Hodkinson, Trevor/0000-0003-1384-7270; Barth, Susanne/0000-0002-4104-5964 FU Teagasc 'Vision' programme; Teagasc Walsh Fellowship Scheme; Irish Department of Agriculture, Food and the Marine (DAFM) FX We thank Choun-Sea Lin who released the two bamboo sequences to us prior to their publication. We thank Sarah McGrath for sharing DNA from L. perenne populations. This work was part of the PhD thesis of the first author (K. D.) and was supported by the Teagasc 'Vision' programme. K. D. was financed under the Teagasc Walsh Fellowship Scheme. Partial funding of this work was obtained from the Irish Department of Agriculture, Food and the Marine (DAFM) under the 'Genetic Resources Fund for Food and Agriculture'. NR 53 TC 7 Z9 7 U1 5 U2 45 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0305-7364 J9 ANN BOT-LONDON JI Ann. Bot. PD NOV PY 2012 VL 110 IS 6 BP 1327 EP 1339 DI 10.1093/aob/mcs044 PG 13 WC Plant Sciences SC Plant Sciences GA 027RV UT WOS:000310371800023 PM 22419761 ER PT J AU Nielsen, CE Wilson, DA Brooks, AL McCord, SL Dagle, GE James, AC Tolmachev, SY Thrall, BD Morgan, WF AF Nielsen, Christopher E. Wilson, Dulaney A. Brooks, Antone L. McCord, Stacey L. Dagle, Gerald E. James, Anthony C. Tolmachev, Sergei Y. Thrall, Brian D. Morgan, William F. TI Microdistribution and Long-term Retention of Pu-239 (NO3)(4) in the Respiratory Tracts of an Acutely Exposed Plutonium Worker and Experimental Beagle Dogs SO CANCER RESEARCH LA English DT Article ID LIVER AB The long-term retention of inhaled soluble forms of plutonium raises concerns as to the potential health effects in persons working in nuclear energy or the nuclear weapons program. The distributions of long-term retained inhaled plutonium-nitrate [Pu-239 (NO3)(4)] deposited in the lungs of an accidentally exposed nuclear worker (Human Case 0269) and in the lungs of experimentally exposed beagle dogs with varying initial lung depositions were determined via autoradiographs of selected histologic lung, lymph node, trachea, and nasal turbinate tissue sections. These studies showed that both the human and dogs had a nonuniform distribution of plutonium throughout the lung tissue. Fibrotic scar tissue effectively encapsulated a portion of the plutonium and prevented its clearance from the body or translocation to other tissues and diminished dose to organ parenchyma. Alpha radiation activity from deposited plutonium in Human Case 0269 was observed primarily along the subpleural regions while no alpha activity was seen in the tracheobronchial lymph nodes of this individual. However, relatively high activity levels in the tracheobronchial lymph nodes of the beagles indicated the lymphatic system was effective in clearing deposited plutonium from the lung tissues. In both the human case and beagle dogs, the appearance of retained plutonium within the respiratory tract was inconsistent with current biokinetic models of clearance for soluble forms of plutonium. Bound plutonium can have a marked effect on the dose to the lungs and subsequent radiation exposure has the potential to increase cancer risk. Cancer Res; 72(21); 5529-36. (C)2012 AACR. C1 [Nielsen, Christopher E.; Wilson, Dulaney A.; Brooks, Antone L.; Dagle, Gerald E.; Thrall, Brian D.; Morgan, William F.] Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99352 USA. [McCord, Stacey L.; James, Anthony C.; Tolmachev, Sergei Y.] Washington State Univ, US Transuranium Registry, Richland, WA USA. [McCord, Stacey L.; James, Anthony C.; Tolmachev, Sergei Y.] Washington State Univ, Uranium Registry, Richland, WA USA. RP Nielsen, CE (reprint author), Pacific NW Natl Lab, Div Biol Sci, 902 Battelle Blvd,POB 999,MSIN J4-02, Richland, WA 99352 USA. EM christopher.nielsen@pnnl.gov RI Tolmachev, Sergei/C-1397-2011; WSU, USTUR/I-1056-2013; OI Tolmachev, Sergei/0000-0003-0077-106X; Wilson, Dulaney/0000-0003-4726-7848 FU Laboratory Directed Research Development award from the Pacific Northwest National Laboratory; Battelle Memorial Institute; Pacific Northwest Division under U.S. Department of Energy, Office of Biological and Environmental Research Low Dose Science Program [DE-AC05-76RL0 1830]; Fred Hutchinson Cancer Research Center, National Institute for Allergy and Infectious Disease [U19 AI 067770]; U.S. Department of Energy, Office of Injury and Illness Prevention Programs [HS-13, DE-FG06-92EH89181] FX This study was supported by a Laboratory Directed Research Development award from the Pacific Northwest National Laboratory, the Battelle Memorial Institute, Pacific Northwest Division, under Contract No. DE-AC05-76RL0 1830 with the U.S. Department of Energy, Office of Biological and Environmental Research Low Dose Science Program, and a pilot award from the Fred Hutchinson Cancer Research Center, National Institute for Allergy and Infectious Disease grant U19 AI 067770, Center for Medical Countermeasures against Radiation. The USTUR is funded by U.S. Department of Energy, Office of Injury and Illness Prevention Programs (HS-13), under Grant Award No.: DE-FG06-92EH89181. NR 19 TC 5 Z9 6 U1 1 U2 17 PU AMER ASSOC CANCER RESEARCH PI PHILADELPHIA PA 615 CHESTNUT ST, 17TH FLOOR, PHILADELPHIA, PA 19106-4404 USA SN 0008-5472 J9 CANCER RES JI Cancer Res. PD NOV 1 PY 2012 VL 72 IS 21 BP 5529 EP 5536 DI 10.1158/0008-5472.CAN-12-1824 PG 8 WC Oncology SC Oncology GA 030PG UT WOS:000310582000011 PM 22962267 ER PT J AU Okumura, K Sato, M Saito, M Miura, I Wakana, S Mao, JH Miyasaka, Y Kominami, R Wakabayashi, Y AF Okumura, Kazuhiro Sato, Miho Saito, Megumi Miura, Ikuo Wakana, Shigeharu Mao, Jian-Hua Miyasaka, Yuki Kominami, Ryo Wakabayashi, Yuichi TI Independent genetic control of early and late stages of chemically induced skin tumors in a cross of a Japanese wild-derived inbred mouse strain, MSM/Ms SO CARCINOGENESIS LA English DT Article ID CANCER SUSCEPTIBILITY LOCUS; CONGENIC STRAINS; LUNG-CANCER; MICE; IDENTIFICATION; RESISTANCE; CANDIDATE; PROMOTION; MODELS; LYMPHOMA AB MSM/Ms is an inbred mouse strain derived from a Japanese wild mouse, Mus musculus molossinus. In this study, we showed that MSM/Ms mice exhibit dominant resistance when crossed with susceptible FVB/N mice and subjected to the two-stage skin carcinogenesis protocol using 7,12-dimethylbenz(a)anthracene (DMBA)/12-O-tetradecanoylphorbol-13-acetate (TPA). A series of F1 backcross mice were generated by crossing p53(+/+) or p53(+/-) F1 (FVB/N x MSM/Ms) males with FVB/N female mice. These generated 228 backcross animals, approximately half of which were p53(+/-), enabling us to search for p53-dependent skin tumor modifier genes. Highly significant linkage for papilloma multiplicity was found on chromosomes 6 and 7 and suggestive linkage was found on chromosomes 3, 5 and 12. Furthermore, in order to identify stage-dependent linkage loci we classified tumors into three categories (<2 mm, 2-6 mm and >6 mm), and did linkage analysis. The same locus on chromosome 7 showed strong linkage in groups with <2 mm or 2-6 mm papillomas. No linkage was detected on chromosome 7 to papillomas >6 mm, but a different locus on chromosome 4 showed strong linkage both to papillomas >6 mm and to carcinomas. This locus, which maps near the Cdkn2a/p19(Arf) gene, was entirely p53-dependent, and was not seen in p53(+/-) backcross animals. Suggestive linkage conferring susceptibility to carcinoma was also found on chromosome 5. These results clearly suggest distinct loci regulate each stage of tumorigenesis, some of which are p53-dependent. C1 [Okumura, Kazuhiro; Sato, Miho; Saito, Megumi; Wakabayashi, Yuichi] Chiba Canc Ctr, Res Inst, Div Expt Anim Res, Dept Carcinogenesis Res,Chuou Ku, Chiba 2608717, Japan. [Okumura, Kazuhiro; Sato, Miho; Wakabayashi, Yuichi] Niigata Univ, Lab Genet Mech, Grad Sch Med & Dent Sci, Niigata 9518510, Japan. [Miura, Ikuo; Wakana, Shigeharu] Riken Bioresource Ctr, Technol & Dev Team Mouse Phenotype Analysis Japan, Tsukuba, Ibaraki 3050074, Japan. [Mao, Jian-Hua] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. [Miyasaka, Yuki; Kominami, Ryo] Niigata Univ, Grad Sch Med & Dent Sci, Dept Mol Genet, Niigata 9518510, Japan. RP Wakabayashi, Y (reprint author), Chiba Canc Ctr, Res Inst, Div Expt Anim Res, Dept Carcinogenesis Res,Chuou Ku, 666-2 Nitonacho, Chiba 2608717, Japan. EM yuichi_wakabayashi@chiba-cc.jp FU MEXT's program "Promotion of Environmental Improvement for Independence of Young Researchers" under the Special Coordination Funds for Promoting Science and Technology at Niigata University FX MEXT's program "Promotion of Environmental Improvement for Independence of Young Researchers" under the Special Coordination Funds for Promoting Science and Technology at Niigata University. NR 42 TC 4 Z9 4 U1 0 U2 1 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0143-3334 J9 CARCINOGENESIS JI Carcinogenesis PD NOV PY 2012 VL 33 IS 11 BP 2260 EP 2268 DI 10.1093/carcin/bgs250 PG 9 WC Oncology SC Oncology GA 031FL UT WOS:000310624400029 PM 22843548 ER PT J AU Baker, LR Kennedy, G Krier, JM Van Spronsen, M Onorato, RM Somorjai, GA AF Baker, L. Robert Kennedy, Griffin Krier, James M. Van Spronsen, Matthijs Onorato, Robert M. Somorjai, Gabor A. TI The Role of an Organic Cap in Nanoparticle Catalysis: Reversible Restructuring of Carbonaceous Material Controls Catalytic Activity of Platinum Nanoparticles for Ethylene Hydrogenation and Methanol Oxidation SO CATALYSIS LETTERS LA English DT Article DE Capping agent; Nanoparticles; Nanotechnology; SFG; Microscopy; Spectroscopy and general characterisation; Heterogeneous catalysis; Catalysis ID SUM-FREQUENCY GENERATION; MESOPOROUS SBA-15 SILICA; VIBRATIONAL SPECTROSCOPY; STRUCTURE SENSITIVITY; CRYSTAL-SURFACES; CO DISSOCIATION; GAS-PHASE; SIZE; SELECTIVITY; SHAPE AB Inherent in the colloidal synthesis of nanoparticle catalysts is the presence of an organic capping agent that encapsulates the nanoparticles to prevent aggregation. However, this capping agent often remains present on the nanoparticles during catalytic reaction, and the effect of this coating on catalysis is an important question that will influence the future applications of colloidal nanoparticles. In this study, the structure of poly(vinylpyrrolidone) (PVP) ligands on Pt nanoparticles is probed using sum frequency generation vibrational spectroscopy before and after cap removal by UV light. When the PVP is removed, carbonaceous fragments remain on the surface that dynamically restructure in H-2 and O-2. These fragments form a porous coating around the Pt in H-2 but collapse to a tightly closed shell in O-2. Using ethylene hydrogenation and methanol oxidation as a probe for the catalytic activity of the nanoparticles in H-2 and O-2, respectively, it is shown that the structure of these carbonaceous fragments controls the catalytic activity of the nanoparticles across several orders of magnitude by opening in H-2 and collapsing to block Pt sites in O-2. Kinetic experiments on thermally-cleaned PVP-capped and oleic acid-capped nanoparticles show that these findings apply to multiple capping agents and cleaning methods. This work highlights the dominant role of an organic cap to mediate nanoparticle catalysis and provides one example where capped nanoparticles are dramatically better catalysts than their uncapped analogues. C1 [Baker, L. Robert; Kennedy, Griffin; Krier, James M.; Onorato, Robert M.; Somorjai, Gabor A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Baker, L. Robert; Kennedy, Griffin; Krier, James M.; Onorato, Robert M.; Somorjai, Gabor A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem, Berkeley, CA 94720 USA. [Baker, L. Robert; Kennedy, Griffin; Krier, James M.; Onorato, Robert M.; Somorjai, Gabor A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Van Spronsen, Matthijs] Leiden Univ, Leiden Inst Chem, NL-2300 RA Leiden, Netherlands. RP Baker, LR (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM lrbaker@berkeley.edu; somorjai@berkeley.edu FU Helios Solar Energy Research Center; Chemical and Materials Sciences Divisions; Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was funded by the Helios Solar Energy Research Center and by the Chemical and Materials Sciences Divisions, which are supported by the Director, Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 34 TC 21 Z9 21 U1 6 U2 112 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1011-372X J9 CATAL LETT JI Catal. Lett. PD NOV PY 2012 VL 142 IS 11 BP 1286 EP 1294 DI 10.1007/s10562-012-0904-3 PG 9 WC Chemistry, Physical SC Chemistry GA 032UK UT WOS:000310744400003 ER PT J AU Di Pierro, M Skinner, D AF Di Pierro, Massimo Skinner, David TI Concurrency in Modern Programming Languages SO COMPUTING IN SCIENCE & ENGINEERING LA English DT Editorial Material C1 [Di Pierro, Massimo] Depaul Univ, Sch Comp Digital Media, Chicago, IL 60604 USA. [Skinner, David] Lawrence Berkeley Natl Lab, Sci Discovery Adv Comp SciDAC Outreach Ctr, Berkeley, CA USA. RP Di Pierro, M (reprint author), Depaul Univ, Sch Comp Digital Media, Chicago, IL 60604 USA. EM mdipierro@cs.depaul.edu; deskinner@lbl.gov NR 0 TC 1 Z9 1 U1 0 U2 2 PU IEEE COMPUTER SOC PI LOS ALAMITOS PA 10662 LOS VAQUEROS CIRCLE, PO BOX 3014, LOS ALAMITOS, CA 90720-1314 USA SN 1521-9615 J9 COMPUT SCI ENG JI Comput. Sci. Eng. PD NOV-DEC PY 2012 VL 14 IS 6 BP 8 EP 10 PG 3 WC Computer Science, Interdisciplinary Applications SC Computer Science GA 025UU UT WOS:000310221500002 ER PT J AU Landis, DD Hummelshoj, JS Nestorov, S Greeley, J Dulak, M Bligaard, T Norskov, JK Jacobsen, KW AF Landis, David D. Hummelshoj, Jens S. Nestorov, Svetlozar Greeley, Jeff Dulak, Marcin Bligaard, Thomas Norskov, Jens K. Jacobsen, Karsten W. TI The Computational Materials Repository SO COMPUTING IN SCIENCE & ENGINEERING LA English DT Article AB The possibilities for designing new materials based on quantum physics calculations are rapidly growing, but these design efforts lead to a significant increase in the amount of computational data created. The Computational Materials Repository (CMR) addresses this data challenge and provides a software infrastructure that supports the collection, storage, retrieval, analysis, and sharing of data produced by many electronic-structure simulators. C1 [Landis, David D.] Tech Univ Denmark, Ctr Atom Scale Mat Design CAMD, Dept Phys, Lyngby, Denmark. [Hummelshoj, Jens S.; Bligaard, Thomas; Norskov, Jens K.] Stanford Univ, Stanford, CA 94305 USA. [Nestorov, Svetlozar] Univ Chicago, Computat Inst, Chicago, IL 60637 USA. [Greeley, Jeff] Argonne Natl Lab, Theory & Modeling Grp, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Jacobsen, Karsten W.] Tech Univ Denmark, CAMD, Lyngby, Denmark. RP Landis, DD (reprint author), Tech Univ Denmark, Ctr Atom Scale Mat Design CAMD, Dept Phys, Lyngby, Denmark. EM dlandis@fysik.dtu.dk; strabo@slac.stanford.edu; evtimov@cs.uchicago.edu; jgreeley@anl.gov; Marcin.Dulak@fysik.dtu.dk; bligaard@stanford.edu; norskov@stanford.edu; kwj@fysik.dtu.dk RI Bligaard, Thomas/A-6161-2011; Jacobsen, Karsten/B-3602-2009; Norskov, Jens/D-2539-2017 OI Bligaard, Thomas/0000-0001-9834-9179; Jacobsen, Karsten/0000-0002-1121-2979; Norskov, Jens/0000-0002-4427-7728 FU Danish Center for Scientific Computing; Danish Council for Strategic Research's Programme Commission on Nanoscience, Nanotechnology, Biotechnology, and IT (NABIIT); Lundbeck Foundation; US Department of Energy (DOE); Department of Energy, Office of Science; Office of Basic Energy Sciences through the Early Career Research Program FX We acknowledge financial support from the Danish Center for Scientific Computing and the Danish Council for Strategic Research's Programme Commission on Nanoscience, Nanotechnology, Biotechnology, and IT (NABIIT). The Center for Atomic-Scale Materials Design (CAMD) is funded by the Lundbeck Foundation. The Sustainable Energy through Catalysis (Suncat) Center for Interface Science and Catalysis is funded by the US Department of Energy (DOE). Jeff Greeley acknowledges support from the Department of Energy, Office of Science, and Office of Basic Energy Sciences through the Early Career Research Program. NR 4 TC 27 Z9 27 U1 6 U2 64 PU IEEE COMPUTER SOC PI LOS ALAMITOS PA 10662 LOS VAQUEROS CIRCLE, PO BOX 3014, LOS ALAMITOS, CA 90720-1314 USA SN 1521-9615 J9 COMPUT SCI ENG JI Comput. Sci. Eng. PD NOV-DEC PY 2012 VL 14 IS 6 BP 51 EP 57 PG 7 WC Computer Science, Interdisciplinary Applications SC Computer Science GA 025UU UT WOS:000310221500007 ER PT J AU Grinberg, L Insley, JA Fedosov, DA Morozov, V Papka, ME Karniadakis, GE AF Grinberg, Leopold Insley, Joseph A. Fedosov, Dmitry A. Morozov, Vitali Papka, Michael E. Karniadakis, George Em TI TIGHTLY COUPLED ATOMISTIC-CONTINUUM SIMULATIONS OF BRAIN BLOOD FLOW ON PETAFLOP SUPERCOMPUTERS SO COMPUTING IN SCIENCE & ENGINEERING LA English DT Article ID DISSIPATIVE PARTICLE DYNAMICS AB Several advances on the mathematical, computational, and visualization fronts have led to the first truly multiscale simulation and visualization of a realistic biological system. C1 [Grinberg, Leopold] Brown Univ, Div Appl Math, Providence, RI 02912 USA. [Insley, Joseph A.] Univ Chicago, Chicago, IL 60637 USA. [Insley, Joseph A.; Papka, Michael E.] Argonne Natl Lab, Argonne, IL 60439 USA. [Fedosov, Dmitry A.] Forschungszentrum Julich, Inst Complex Syst, D-52425 Julich, Germany. [Papka, Michael E.] No Illinois Univ, De Kalb, IL 60115 USA. [Karniadakis, George Em] MIT, Cambridge, MA 02139 USA. RP Grinberg, L (reprint author), Brown Univ, Div Appl Math, Providence, RI 02912 USA. EM leopold_grinberg@brown.edu; insley@anl.gov; d.fedosov@fz-juelich.de; morozov@anl.gov; papka@anl.gov; gk@dam.brown.edu RI Fedosov, Dmitry/G-4110-2013 OI Fedosov, Dmitry/0000-0001-7469-9844 FU US Department of Energy's Innovative and Novel Computational Impact on Theory and Experiment (INCITE) grant [DE-AC02-06CH11357]; National Science Foundation [OCI-0636336, OCI-0904190] FX Computations were performed on the IBM Blue Gene/P computer of Argonne National Laboratory and the Julich Supercomputing Centre, along with the Cray XT5 computer of the US National Institute for Computational Sciences and Oak Ridge National Laboratory. The visualization was performed on Eureka at the Argonne Leadership Computing Facility. Support was provided by the US Department of Energy's Innovative and Novel Computational Impact on Theory and Experiment (INCITE) grant DE-AC02-06CH11357, as well as National Science Foundation grants OCI-0636336 and OCI-0904190. NR 14 TC 4 Z9 5 U1 0 U2 16 PU IEEE COMPUTER SOC PI LOS ALAMITOS PA 10662 LOS VAQUEROS CIRCLE, PO BOX 3014, LOS ALAMITOS, CA 90720-1314 USA SN 1521-9615 J9 COMPUT SCI ENG JI Comput. Sci. Eng. PD NOV-DEC PY 2012 VL 14 IS 6 BP 58 EP 67 PG 10 WC Computer Science, Interdisciplinary Applications SC Computer Science GA 025UU UT WOS:000310221500008 ER PT J AU Chen, L Wang, Y AF Chen, Ling Wang, Yang TI Heat Map Displays for Data From Human Abuse Potential Crossover Studies SO DRUG INFORMATION JOURNAL LA English DT Article DE drug abuse potential; crossover study; graphic method; heat map; Williams square design ID LIABILITY AB The human abuse potential study is an important part of the assessment of abuse potential of drugs. This type of study has multiple treatments and multiple abuse potential measures. The study is crossover and often uses a Williams square design. Data are collected for treatments from each treatment sequence and during each treatment period at many time points. This article proposes the use of heat maps to display complicated data sets. This graphic method provides a visual tool for exploring data from individual subjects and overall pictures of subject responses in human abuse potential studies. C1 [Chen, Ling; Wang, Yang] US FDA, ORISE, Ctr Drug Evaluat & Res, Silver Spring, MD 20993 USA. RP Chen, L (reprint author), US FDA, ORISE, Ctr Drug Evaluat & Res, 10903 New Hampshire Ave,White Oak Bldg 21,Room 46, Silver Spring, MD 20993 USA. EM ling.chen@fda.hhs.gov FU Regulatory Science Review Enhancement Program; Controlled Substance Staff (CSS) at the Center for Drug Evaluation and Research, US Food and Drug Administration FX This research was supported by funding from the Regulatory Science Review Enhancement Program as well as the Controlled Substance Staff (CSS) at the Center for Drug Evaluation and Research, US Food and Drug Administration. NR 10 TC 0 Z9 0 U1 3 U2 6 PU SAGE PUBLICATIONS INC PI THOUSAND OAKS PA 2455 TELLER RD, THOUSAND OAKS, CA 91320 USA SN 0092-8615 J9 DRUG INF J JI Drug Inf. J. PD NOV PY 2012 VL 46 IS 6 BP 701 EP 707 DI 10.1177/0092861512452120 PG 7 WC Health Care Sciences & Services; Pharmacology & Pharmacy SC Health Care Sciences & Services; Pharmacology & Pharmacy GA 032HF UT WOS:000310705100011 ER PT J AU Schwartz, YB Linder-Basso, D Kharchenko, PV Tolstorukov, MY Kim, M Li, HB Gorchakov, AA Minoda, A Shanower, G Alekseyenko, AA Riddle, NC Jung, YL Gu, TT Plachetka, A Elgin, SCR Kuroda, MI Park, PJ Savitsky, M Karpen, GH Pirrotta, V AF Schwartz, Yuri B. Linder-Basso, Daniela Kharchenko, Peter V. Tolstorukov, Michael Y. Kim, Maria Li, Hua-Bing Gorchakov, Andrey A. Minoda, Aki Shanower, Gregory Alekseyenko, Artyom A. Riddle, Nicole C. Jung, Youngsook L. Gu, Tingting Plachetka, Annette Elgin, Sarah C. R. Kuroda, Mitzi I. Park, Peter J. Savitsky, Mikhail Karpen, Gary H. Pirrotta, Vincenzo TI Nature and function of insulator protein binding sites in the Drosophila genome SO GENOME RESEARCH LA English DT Article ID RESPONSE ELEMENT PRE; ZINC-FINGER PROTEIN; CHROMATIN INSULATOR; GENE-EXPRESSION; ENHANCER BLOCKING; CTCF-BINDING; SUPPRESSOR; POLYCOMB; GYPSY; MELANOGASTER AB Chromatin insulator elements and associated proteins have been proposed to partition eukaryotic genomes into sets of independently regulated domains. Here we test this hypothesis by quantitative genome-wide analysis of insulator protein binding to Drosophila chromatin. We find distinct combinatorial binding of insulator proteins to different classes of sites and uncover a novel type of insulator element that binds CP190 but not any other known insulator proteins. Functional characterization of different classes of binding sites indicates that only a small fraction act as robust insulators in standard enhancer-blocking assays. We show that insulators restrict the spreading of the H3K27me3 mark but only at a small number of Polycomb target regions and only to prevent repressive histone methylation within adjacent genes that are already transcriptionally inactive. RNAi knockdown of insulator proteins in cultured cells does not lead to major alterations in genome expression. Taken together, these observations argue against the concept of a genome partitioned by specialized boundary elements and suggest that insulators are reserved for specific regulation of selected genes. C1 [Schwartz, Yuri B.; Kim, Maria; Savitsky, Mikhail] Umea Univ, Dept Mol Biol, S-90187 Umea, Sweden. [Schwartz, Yuri B.; Linder-Basso, Daniela; Li, Hua-Bing; Shanower, Gregory; Pirrotta, Vincenzo] Rutgers State Univ, Dept Mol Biol & Biochem, Piscataway, NJ 08901 USA. [Kharchenko, Peter V.; Tolstorukov, Michael Y.; Jung, Youngsook L.; Park, Peter J.] Harvard Univ, Sch Med, Ctr Biomed Informat, Boston, MA 02115 USA. [Kim, Maria; Savitsky, Mikhail] Inst Gene Biol, Grp Telomere Biol, Moscow 119334, Russia. [Gorchakov, Andrey A.; Alekseyenko, Artyom A.; Plachetka, Annette; Kuroda, Mitzi I.] Brigham & Womens Hosp, Dept Med, Div Genet, Boston, MA 02115 USA. [Gorchakov, Andrey A.; Alekseyenko, Artyom A.; Plachetka, Annette; Kuroda, Mitzi I.] Harvard Univ, Sch Med, Dept Genet, Boston, MA 02115 USA. [Gorchakov, Andrey A.] Inst Mol & Cellular Biol, Novosibirsk 630090, Russia. [Minoda, Aki; Karpen, Gary H.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Minoda, Aki; Karpen, Gary H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Genome Dynam, Berkeley, CA 94720 USA. [Riddle, Nicole C.; Gu, Tingting; Elgin, Sarah C. R.] Washington Univ, Dept Biol, St Louis, MO 63130 USA. RP Schwartz, YB (reprint author), Umea Univ, Dept Mol Biol, S-90187 Umea, Sweden. EM yuri.schwartz@molbiol.umu.se; pirrotta@biology.rutgers.edu RI Li, Huabing/M-5390-2013; Gorchakov, Andrey/N-5840-2015; Minoda, Aki/D-5335-2017 OI Li, Huabing/0000-0003-3573-6803; Gorchakov, Andrey/0000-0003-2830-4236; Minoda, Aki/0000-0002-2927-5791 FU NIH modENCODE grant [U01HG004258]; Wenner-Gren Foundations; Russian Academy of Sciences FX We thank D. Acevedo, S. Gadel, C. Kennedy, and Rutgers BRTC for excellent technical assistance. We thank R. Renkawitz, V. Corces, F. Karch, R. Dorn, and S. Small for generous gifts of antibodies, fly stocks, and plasmids. This work was supported by NIH modENCODE grant U01HG004258 (G. H. K., M. I. K., P.J.P., S. C. R. E., V. P.), Wenner-Gren Foundations (Y.B.S.), and the Russian Academy of Sciences program for Molecular and Cellular Biology (M.S.). NR 44 TC 71 Z9 72 U1 0 U2 13 PU COLD SPRING HARBOR LAB PRESS, PUBLICATIONS DEPT PI COLD SPRING HARBOR PA 1 BUNGTOWN RD, COLD SPRING HARBOR, NY 11724 USA SN 1088-9051 J9 GENOME RES JI Genome Res. PD NOV PY 2012 VL 22 IS 11 BP 2188 EP 2198 DI 10.1101/gr.138156.112 PG 11 WC Biochemistry & Molecular Biology; Biotechnology & Applied Microbiology; Genetics & Heredity SC Biochemistry & Molecular Biology; Biotechnology & Applied Microbiology; Genetics & Heredity GA 030QE UT WOS:000310584400011 PM 22767387 ER PT J AU Rampe, EB Kraft, MD Sharp, TG Golden, DC Ming, DW Christensen, PR AF Rampe, E. B. Kraft, M. D. Sharp, T. G. Golden, D. C. Ming, D. W. Christensen, P. R. TI Allophane detection on Mars with Thermal Emission Spectrometer data and implications for regional-scale chemical weathering processes SO GEOLOGY LA English DT Article ID MARTIAN SURFACE; SYNTHETIC ALLOPHANE; MERIDIANI-PLANUM; ICE DEPOSITS; MINERALOGY; COMPONENT; SPECTRA; BASALT; TES AB Models of Thermal Emission Spectrometer (TES) data suggest that poorly-crystalline weathering products allophane and aluminosilicate gel occur in several low-albedo regions of Mars. The presence of allophane in TES models indicates that the martian surface experienced low-temperature chemical weathering at low water-to-rock ratios and mildly acidic to neutral pH on regional scales. The allophane and gel may be ancient and preserved by a persistently dry martian climate. Alternatively, evidence for recent ground ice in these regions suggests that pedogenic processes causing the formation of poorly-crystalline aluminosilicates could be late Amazonian in age and may be active today. While previous models have suggested that global-scale acidic weathering has occurred on Mars for the past 3.5 billion years, the presence of allophane indicates that acidic weathering was not occurring in these low-albedo regions and that mildly acidic to neutral weathering has been an important regional-scale weathering process on the martian surface. C1 [Rampe, E. B.; Ming, D. W.] NASA, Lyndon B Johnson Space Ctr, Houston, TX 77058 USA. [Rampe, E. B.] Oak Ridge Associated Univ, Oak Ridge, TN 37831 USA. [Kraft, M. D.; Sharp, T. G.; Christensen, P. R.] Arizona State Univ, Sch Earth & Space Explorat, Tempe, AZ 85287 USA. [Golden, D. C.] Engn & Sci Contract Grp Hamilton Sundstrand, Houston, TX 77058 USA. RP Rampe, EB (reprint author), NASA, Lyndon B Johnson Space Ctr, Houston, TX 77058 USA. EM elizabeth.b.rampe@nasa.gov FU NASA [NNX07AP11H] FX We thank A.D. Rogers for her input and insight. We thank J. Quinn for quantifying allophane compositions. We gratefully acknowledge the use of facilities within the LeRoy Eyring Center for Solid State Science at Arizona State University. This manuscript was improved by helpful reviews by M. McDowell and two anonymous reviewers. This research was supported by NASA Graduate Student Researchers Program grant NNX07AP11H. NR 29 TC 13 Z9 13 U1 0 U2 15 PU GEOLOGICAL SOC AMER, INC PI BOULDER PA PO BOX 9140, BOULDER, CO 80301-9140 USA SN 0091-7613 EI 1943-2682 J9 GEOLOGY JI Geology PD NOV PY 2012 VL 40 IS 11 BP 995 EP 998 DI 10.1130/G33215.1 PG 4 WC Geology SC Geology GA 028GO UT WOS:000310411000009 ER PT J AU Korom, SF Seaman, JC AF Korom, Scott F. Seaman, John C. TI When "Conservative" Anionic Tracers Aren't SO GROUND WATER LA English DT Article ID HETEROGENEOUS AQUIFER; ADSORPTION; DISPERSION; CHLORIDE; BROMIDE; MEDIA; FIELD; RETARDATION; EXCLUSION; MIGRATION C1 [Korom, Scott F.] Univ N Dakota, Dept Geol & Geol Engn, Grand Forks, ND 58202 USA. [Seaman, John C.] Univ Georgia, Savannah River Ecol Lab, Aiken, SC 29802 USA. RP Korom, SF (reprint author), Univ N Dakota, Dept Geol & Geol Engn, 81 Cornell Stop 8358, Grand Forks, ND 58202 USA. EM scott.korom@engr.und.edu FU Savannah River Ecology Laboratory from the Department of Energy [DE-FC09-07SR22506] FX S.F.K. contributed to this technical commentary while on developmental leave from the University of North Dakota. J.C.S.'s participation was supported by the Savannah River Ecology Laboratory through Financial Assistance Award DE-FC09-07SR22506 from the Department of Energy to the University of Georgia Research Foundation. The comments of three anonymous reviewers improved our manuscript. NR 24 TC 4 Z9 4 U1 1 U2 21 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0017-467X J9 GROUND WATER JI Ground Water PD NOV-DEC PY 2012 VL 50 IS 6 BP 820 EP 824 DI 10.1111/j.1745-6584.2012.00950.x PG 5 WC Geosciences, Multidisciplinary; Water Resources SC Geology; Water Resources GA 032OR UT WOS:000310729100002 PM 22582871 ER PT J AU Nlebedim, IC Snyder, JE Moses, AJ Jiles, DC AF Nlebedim, I. C. Snyder, J. E. Moses, A. J. Jiles, D. C. TI Anisotropy and Magnetostriction in Non-Stoichiometric Cobalt Ferrite SO IEEE TRANSACTIONS ON MAGNETICS LA English DT Article; Proceedings Paper CT International Magnetics Conference (INTERMAG) CY MAY 07-11, 2012 CL Vancouver, CANADA SP IEEE, Magnet Soc DE Cobalt ferrite; magnetite; magnetocrystalline anisotropy; magnetostriction; non-stoichiometry; strain sensitivity ID MAGNETIC-ANISOTROPY; ORIGIN AB This study shows the effect of deviation from stoichiometric composition on the anisotropy and magnetostriction of cobalt ferrite CoxFe3-xO4. Deviation from stoichiometric composition caused the magnetocrystalline anisotropy to become higher for x = 0.7 and 0.8, but lower for x = 0.2. The amplitude, slope and shape of the magnetostriction curves and strain derivatives of the samples were also strongly affected. The present work indicates how variation from stoichiometric composition can be used to tailor magnetic and magnetostrictive properties. C1 [Nlebedim, I. C.; Jiles, D. C.] US DOE, Ames Lab, Ames, IA 50011 USA. [Snyder, J. E.] Natl Sci Fdn, Arlington, VA 22230 USA. [Snyder, J. E.; Moses, A. J.] Cardiff Univ, Sch Engn, Wolfson Ctr Magnet, Cardiff CF24 3AA, S Glam, Wales. [Jiles, D. C.] Iowa State Univ, Dept Elect & Comp Engn, Ames, IA 50011 USA. RP Nlebedim, IC (reprint author), US DOE, Ames Lab, Ames, IA 50011 USA. NR 20 TC 24 Z9 24 U1 2 U2 38 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0018-9464 EI 1941-0069 J9 IEEE T MAGN JI IEEE Trans. Magn. PD NOV PY 2012 VL 48 IS 11 BP 3084 EP 3087 DI 10.1109/TMAG.2012.2200884 PG 4 WC Engineering, Electrical & Electronic; Physics, Applied SC Engineering; Physics GA 025MV UT WOS:000310194400090 ER PT J AU Vitol, EA Novosad, V Rozhkova, EA AF Vitol, Elina A. Novosad, Valentyn Rozhkova, Elena A. TI Multifunctional Ferromagnetic Disks for Modulating Cell Function SO IEEE TRANSACTIONS ON MAGNETICS LA English DT Article; Proceedings Paper CT International Magnetics Conference (INTERMAG) CY MAY 07-11, 2012 CL Vancouver, CANADA SP IEEE, Magnet Soc DE Biomagnetics; ferromagnetic disks; magnetomechanical cell actuation; hyperthermia; MRI ID FREQUENCY ELECTROMAGNETIC-FIELDS; MECHANOSENSITIVE ION CHANNELS; MAGNETIC PARTICLES; APOPTOSIS; CANCER; MECHANOTRANSDUCTION; NANOPARTICLES; CYTOSKELETON; CONSTRAINTS; PROTOPLASM AB In this work, we focus on the methods for controlling cell function with ferromagnetic disk-shaped particles. We will first review the history of magnetically assisted modulation of cell behavior and applications of magnetic particles for studying physical properties of a cell. Then, we consider the biological applications of the microdisks such as the method for induction of cancer cell apoptosis, controlled drug release, hyperthermia and MRI imaging. C1 [Vitol, Elina A.; Rozhkova, Elena A.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Vitol, Elina A.; Novosad, Valentyn] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Rozhkova, EA (reprint author), Argonne Natl Lab, Ctr Nanoscale Mat, 9700 S Cass Ave, Argonne, IL 60439 USA. EM rozhkova@anl.gov RI Vitol, Elina/G-6395-2012; Novosad, Valentyn/C-2018-2014; Novosad, V /J-4843-2015 FU NINDS NIH HHS [R01 NS077388] NR 46 TC 13 Z9 13 U1 1 U2 36 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0018-9464 J9 IEEE T MAGN JI IEEE Trans. Magn. PD NOV PY 2012 VL 48 IS 11 BP 3269 EP 3274 DI 10.1109/TMAG.2012.2198209 PG 6 WC Engineering, Electrical & Electronic; Physics, Applied SC Engineering; Physics GA 025MV UT WOS:000310194400138 PM 23766544 ER PT J AU Iavarone, M Scarfato, A Bobba, F Longobardi, M Moore, SA Karapetrov, G Yefremenko, V Novosad, V Cucolo, AM AF Iavarone, M. Scarfato, A. Bobba, F. Longobardi, M. Moore, S. A. Karapetrov, G. Yefremenko, V. Novosad, V. Cucolo, A. M. TI Vortex Confinement in Planar Superconductor/Ferromagnet Hybrid Structures SO IEEE TRANSACTIONS ON MAGNETICS LA English DT Article; Proceedings Paper CT International Magnetics Conference (INTERMAG) CY MAY 07-11, 2012 CL Vancouver, CANADA SP IEEE, Magnet Soc DE Critical current; superconducting films; superconductivity flux pinning ID MAGNETIZATION AB We use low temperature magnetic force microscopy and global magnetometry measurements to study the influence of magnetic domains on the Abrikosov vortex pinning in planar superconducting/ferromagnet bilayers. The superconducting/ferromagnet bilayers consist of a 200 nm superconducting Nb film covering a Permalloy film, with an insulating layer in between to avoid proximity effect. The periodic stripe domain in the Permalloy film produces a potential for directing vortex motion in the adjacent superconducting film. We observed an enhancement of vortex pinning by a factor of 3 that occurs in bilayers with a magnetic stripe domains omega approximate to 500 nm, close to the superconducting critical temperature (T/T-c = 0.9). At lower temperatures, when T/T-c = 0.6 the channeled vortex motion and the intrinsic pinning favor vortex avalanches. C1 [Iavarone, M.; Moore, S. A.] Temple Univ, Dept Phys, Philadelphia, PA 19122 USA. [Scarfato, A.; Bobba, F.; Longobardi, M.; Cucolo, A. M.] Univ Salerno, ER Caianiello Phys Dept, I-84084 Fisciano, Italy. [Scarfato, A.; Bobba, F.; Longobardi, M.; Cucolo, A. M.] CNR SPIN, I-84084 Fisciano, Italy. [Karapetrov, G.] Drexel Univ, Dept Phys, Philadelphia, PA 19104 USA. [Yefremenko, V.; Novosad, V.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Iavarone, M (reprint author), Temple Univ, Dept Phys, Philadelphia, PA 19122 USA. EM iavarone@temple.edu RI Scarfato, Alessandro/A-2582-2013; Novosad, Valentyn/C-2018-2014; Moore, Steven/D-1562-2016; Novosad, V /J-4843-2015; Karapetrov, Goran/C-2840-2008 OI Moore, Steven/0000-0002-3956-815X; Karapetrov, Goran/0000-0003-1113-0137 NR 14 TC 4 Z9 4 U1 0 U2 30 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0018-9464 J9 IEEE T MAGN JI IEEE Trans. Magn. PD NOV PY 2012 VL 48 IS 11 BP 3275 EP 3279 DI 10.1109/TMAG.2012.2196793 PG 5 WC Engineering, Electrical & Electronic; Physics, Applied SC Engineering; Physics GA 025MV UT WOS:000310194400139 ER PT J AU Jaramillo, G Chan, ML Milewski, JO Field, RD Horsley, DA AF Jaramillo, Gerardo Chan, Mei-Lin Milewski, John O. Field, Robert D. Horsley, David A. TI Ferrite Scanning Microscope Based on Magnetic Tunnel Junction Sensor SO IEEE TRANSACTIONS ON MAGNETICS LA English DT Article; Proceedings Paper CT International Magnetics Conference (INTERMAG) CY MAY 07-11, 2012 CL Vancouver, CANADA SP IEEE, Magnet Soc DE Ferrite devices; scanning probe microscopy; tunneling magnetoresistance ID STAINLESS-STEEL; ARRAY AB We have developed a scanning magnetic microscope (SMM) based on a magnetic tunneling junction (MTJ) magnetoresistive (MR) sensor. The microscope is based on commercially available components employing two sets of scanning stages and a MTJ sensor. Spatial resolution and noise sensitivity were investigated using two MTJ sensors, one having high spatial resolution and the other low noise but coarser spatial resolution. We present measurements of magnetic field images from ferrite concentration calibration standards and a stainless steel welded specimen both imaged using a magnetoresistive scanning microscope. A sensitivity of similar to 10 mu T/FN was obtained from standards with defined ferrite numbers (FN). This microscope represents a new powerful tool for the characterization and investigations of delta ferrite concentrations in stainless steel welded samples. C1 [Jaramillo, Gerardo] Univ Calif Davis, Dept Elect & Comp Engn, Davis, CA 95616 USA. [Chan, Mei-Lin; Horsley, David A.] Univ Calif Davis, Dept Mech & Aerosp Engn, Davis, CA 95616 USA. [Milewski, John O.; Field, Robert D.] Los Alamos Natl Lab, Los Alamos, NM 87544 USA. RP Jaramillo, G (reprint author), Univ Calif Davis, Dept Elect & Comp Engn, Davis, CA 95616 USA. EM geomartinez@ucdavis.edu RI Horsley, David/K-7243-2013 NR 11 TC 1 Z9 1 U1 0 U2 10 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0018-9464 J9 IEEE T MAGN JI IEEE Trans. Magn. PD NOV PY 2012 VL 48 IS 11 BP 3677 EP 3680 DI 10.1109/TMAG.2012.2196507 PG 4 WC Engineering, Electrical & Electronic; Physics, Applied SC Engineering; Physics GA 025MV UT WOS:000310194400242 ER PT J AU Hadimani, RL Melikhov, Y Schlagel, DL Lograsso, TA Jiles, DC AF Hadimani, R. L. Melikhov, Y. Schlagel, D. L. Lograsso, T. A. Jiles, D. C. TI Study of the Second-Order "Hidden" Phase Transition of the Monoclinic Phase in the Mixed Phase Region of Gd-5(SixGe1-x)(4) SO IEEE TRANSACTIONS ON MAGNETICS LA English DT Article; Proceedings Paper CT International Magnetics Conference (INTERMAG) CY MAY 07-11, 2012 CL Vancouver, CANADA SP IEEE, Magnet Soc DE Arrott plots; first-order phase transition; Gd-5(SixGe1-x)(4); magnetocaloric materials ID TEMPERATURE; FIELD AB Gd-5(SixGe1-x)(4) exhibits a first order phase transition for the compositions 0 < x < 0.575 leading to a magnetic phase transition as well. It is not possible to measure the second order phase (magnetic) transition temperatures of the individual phases with direct measurements. This is because the first order phase transition occurs before the second order phase transition. With modified Arrott plots we have shown previously that it is possible to estimate the second order phase transition of the Gd5Si4-type orthorhombic phase. In this paper we have estimated the second order phase transition temperature of the Gd5Si2Ge2-type monoclinic phase using a single crystal sample of Gd5Si1.5Ge2.5 (0.375) which falls in the mixed phase region of the sample. C1 [Hadimani, R. L.; Jiles, D. C.] Iowa State Univ, Dept Elect & Comp Engn, Ames, IA 50011 USA. [Melikhov, Y.] Cardiff Univ, Wolfson Ctr Magnet, Cardiff CF24 3AA, S Glam, Wales. [Hadimani, R. L.; Schlagel, D. L.; Lograsso, T. A.; Jiles, D. C.] Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. RP Hadimani, RL (reprint author), Iowa State Univ, Dept Elect & Comp Engn, Ames, IA 50011 USA. EM hadimani@iastate.edu OI Hadimani, Ravi/0000-0001-5939-556X NR 16 TC 4 Z9 4 U1 0 U2 8 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0018-9464 J9 IEEE T MAGN JI IEEE Trans. Magn. PD NOV PY 2012 VL 48 IS 11 BP 4070 EP 4073 DI 10.1109/TMAG.2012.2200245 PG 4 WC Engineering, Electrical & Electronic; Physics, Applied SC Engineering; Physics GA 025MV UT WOS:000310194400344 ER PT J AU Li, SD Wang, LL Xu, J Wang, Z Liu, M Lou, J Beguhn, S Nan, TX Xu, F Sun, NX Duh, JG AF Li, Shandong Wang, Lili Xu, Jie Wang, Zeng Liu, Ming Lou, J. Beguhn, S. Nan, Tianxiang Xu, Feng Sun, Nian X. Duh, Jenq-Gong TI Microwave Frequency Performance and High Magnetic Anisotropy of Fe70Co30-B Films Prepared by a Modified Composition Gradient Sputtering SO IEEE TRANSACTIONS ON MAGNETICS LA English DT Article; Proceedings Paper CT International Magnetics Conference (INTERMAG) CY MAY 07-11, 2012 CL Vancouver, CANADA SP IEEE, Magnet Soc DE Composition gradient sputtering; high-frequency ferromagnetic properties; magnetic anisotropy; soft magnetic films (SMFs) ID THIN-FILMS; UNIAXIAL ANISOTROPY; HIGH PERMEABILITY; MULTILAYER FILM; RU UNDERLAYER; FIELD; HETEROSTRUCTURES; GHZ AB A composition gradient sputtering (CGS) method, in which the doping elements have a gradient distribution from one side to another of the sample, was proposed in our previous work [Li SD, et al. Appl. Phys. Lett., 92 (2008) 092501]. An ultra high magnetic anisotropy field over 500 Oe and ferromagnetic frequency over 7 GHz were obtained in as-deposited FeCoHf films by CGS method due to the stress-induced uniaxial magnetic anisotropy. However, the magnetic properties of the CGS samples are non-uniform, showing a location dependence. In this paper, a modified CGS (MCGS) method was proposed to improve the original CGS method. It is revealed that the MCGS method dramatically improves the uniformity of the high-frequency soft magnetic properties of the as-deposited Fe70Co30 - B films. A narrow ferromagnetic resonance frequency (f(FMR)) range around 5.5 GHz (5.2-5.7 GHz) with a deviation less than 10% and high uniaxial magnetic anisotropy field up to 330 Oe were obtained for as-deposited films with 75 mm in length. As Comparison, the f(FMR) of the CGS samples is very inhomogeneous and distribute in a broad range from 3.1 to 6.7 GHz with a large deviation as high as 116%. The evident advantages of MCGS samples, such as high UMA and relatively uniform high-frequency characteristics, suggest that the MCGS Fe70Co30 - B films are particularly in favor of the integration between magnetic films and RF/microwave components. C1 [Li, Shandong; Xu, Jie; Wang, Zeng] Qingdao Univ, Coll Phys Sci, Qingdao 266071, Peoples R China. [Li, Shandong; Wang, Lili] Fujian Normal Univ, Dept Phys, Fuzhou 350007, Peoples R China. [Liu, Ming; Lou, J.; Beguhn, S.; Nan, Tianxiang; Sun, Nian X.] Northeastern Univ, Dept Elect & Comp Engn, Boston, MA 02115 USA. [Liu, Ming] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Xu, Feng] Nanjing Univ Sci & Technol, Dept Mat Sci & Technol, Nanjing 210091, Peoples R China. [Duh, Jenq-Gong] Natl Tsing Hua Univ, Dept Mat Sci & Engn, Hsinchu 30013, Taiwan. RP Li, SD (reprint author), Qingdao Univ, Coll Phys Sci, Qingdao 266071, Peoples R China. EM dylsd007@yahoo.com.cn RI Lou, Jing/B-6762-2009; Liu, Ming/B-4143-2009; Nan, Tianxiang/O-3820-2015; Nan, Tianxiang/A-8020-2016; Sun, Nian Xiang/F-9590-2010 OI Liu, Ming/0000-0002-6310-948X; Sun, Nian Xiang/0000-0002-3120-0094 NR 26 TC 9 Z9 9 U1 0 U2 27 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0018-9464 EI 1941-0069 J9 IEEE T MAGN JI IEEE Trans. Magn. PD NOV PY 2012 VL 48 IS 11 BP 4313 EP 4316 DI 10.1109/TMAG.2012.2202270 PG 4 WC Engineering, Electrical & Electronic; Physics, Applied SC Engineering; Physics GA 025MV UT WOS:000310194400406 ER PT J AU Kypris, O Nlebedim, IC Jiles, DC AF Kypris, O. Nlebedim, I. C. Jiles, D. C. TI Mapping Stress as a Function of Depth at the Surface of Steel Structures Using a Frequency Dependent Magnetic Barkhausen Noise Technique SO IEEE TRANSACTIONS ON MAGNETICS LA English DT Article; Proceedings Paper CT International Magnetics Conference (INTERMAG) CY MAY 07-11, 2012 CL Vancouver, CANADA SP IEEE, Magnet Soc DE Magnetic Barkhausen noise; nondestructive evaluation; stress depth profiling ID METALLIC FERROMAGNETIC MATERIALS; DOMAIN-WALL DYNAMICS AB Profiling of stress as a function of depth is an important tool for nondestructive evaluation and can be used to prevent catastrophic failures in structures. In this work, the underlying theory of a new model for the depth profiling of stress in ferromagnetic structures based on the magnetic Barkhausen method is investigated and commented upon. In the model, a ferromagnetic structure is divided into layers of different stress states. By analysis of the constituent equations it was found that the measured Barkhausen voltage increases as the frequency span increases, for both the one-and the two layer cases. It was also found that two layers with the same amplitude of Barkhausen emission at the origin can be approximated as one layer, provided that the upper and lower depths, as well as the frequency range are identical. C1 [Kypris, O.; Jiles, D. C.] Iowa State Univ, Dept Elect & Comp Engn, Ames, IA 50011 USA. [Nlebedim, I. C.; Jiles, D. C.] US DOE, Ames Lab, Ames, IA 50011 USA. RP Kypris, O (reprint author), Iowa State Univ, Dept Elect & Comp Engn, Ames, IA 50011 USA. EM kypris@iastate.edu RI Kypris, Orfeas/E-7495-2016 OI Kypris, Orfeas/0000-0001-7858-3259 NR 10 TC 8 Z9 8 U1 1 U2 14 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0018-9464 J9 IEEE T MAGN JI IEEE Trans. Magn. PD NOV PY 2012 VL 48 IS 11 BP 4428 EP 4431 DI 10.1109/TMAG.2012.2196792 PG 4 WC Engineering, Electrical & Electronic; Physics, Applied SC Engineering; Physics GA 025MV UT WOS:000310194400436 ER PT J AU Chartrand, R AF Chartrand, Rick TI Nonconvex Splitting for Regularized Low-Rank plus Sparse Decomposition SO IEEE TRANSACTIONS ON SIGNAL PROCESSING LA English DT Article DE Algorithms; compressed sensing; optimization; principal component analysis; video signal processing ID RECONSTRUCTION; MINIMIZATION; ALGORITHM AB We develop new nonconvex approaches for matrix optimization problems involving sparsity. The heart of the methods is a new, nonconvex penalty function that is designed for efficient minimization by means of a generalized shrinkage operation. We apply this approach to the decomposition of video into low rank and sparse components, which is able to separate moving objects from the stationary background better than in the convex case. In the case of noisy data, we add a nonconvex regularization, and apply a splitting approach to decompose the optimization problem into simple, parallelizable components. The nonconvex regularization ameliorates contrast loss, thereby allowing stronger denoising without losing more signal to the residual. C1 Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Chartrand, R (reprint author), Los Alamos Natl Lab, Div Theoret, MS B284, Los Alamos, NM 87545 USA. EM rickc@lanl.gov OI Chartrand, Rick/0000-0003-3256-2238 FU U.S. Department of Energy through the LANL/LDRD Program FX The author gratefully acknowledges the support of the U.S. Department of Energy through the LANL/LDRD Program for this work. NR 21 TC 30 Z9 34 U1 4 U2 22 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 1053-587X EI 1941-0476 J9 IEEE T SIGNAL PROCES JI IEEE Trans. Signal Process. PD NOV PY 2012 VL 60 IS 11 BP 5810 EP 5819 DI 10.1109/TSP.2012.2208955 PG 10 WC Engineering, Electrical & Electronic SC Engineering GA 024WB UT WOS:000310139900016 ER PT J AU Simon, H Dongarra, J Shukla, H AF Simon, Horst Dongarra, Jack Shukla, Hemant TI Special Issue: Manycore and Accelerator-based High-performance Scientific Computing Introduction SO INTERNATIONAL JOURNAL OF HIGH PERFORMANCE COMPUTING APPLICATIONS LA English DT Editorial Material C1 [Simon, Horst] Lawrence Berkeley Natl Lab, Berkeley Lab, Berkeley, CA USA. [Simon, Horst] Berkeley Lab, Computat Res Div, Berkeley, CA USA. [Simon, Horst] Univ Calif Berkeley, Coll Engn, Berkeley, CA 94720 USA. [Dongarra, Jack] Argonne Natl Lab, Argonne, IL 60439 USA. [Dongarra, Jack] Univ Tennessee, Dept Comp Sci, Knoxville, TN 37996 USA. [Dongarra, Jack] Univ Manchester, Manchester M13 9PL, Lancs, England. [Dongarra, Jack] Rice Univ, Dept Comp Sci, Houston, TX 77251 USA. [Dongarra, Jack] Univ Tennessee, Innovat Comp Lab, Knoxville, TN 37996 USA. [Dongarra, Jack] Univ Tennessee, Ctr Informat Technol Res, Knoxville, TN 37996 USA. [Shukla, Hemant] CALTECH, Space Telescope Sci Inst, Pasadena, CA 91125 USA. [Shukla, Hemant] Stanford Res Syst, Stanford, CA USA. RP Simon, H (reprint author), Lawrence Berkeley Natl Lab, Berkeley Lab, Berkeley, CA USA. RI Dongarra, Jack/E-3987-2014 NR 0 TC 0 Z9 0 U1 0 U2 6 PU SAGE PUBLICATIONS LTD PI LONDON PA 1 OLIVERS YARD, 55 CITY ROAD, LONDON EC1Y 1SP, ENGLAND SN 1094-3420 J9 INT J HIGH PERFORM C JI Int. J. High Perform. Comput. Appl. PD NOV PY 2012 VL 26 IS 4 SI SI BP 335 EP 336 DI 10.1177/1094342012464425 PG 2 WC Computer Science, Hardware & Architecture; Computer Science, Interdisciplinary Applications; Computer Science, Theory & Methods SC Computer Science GA 033KZ UT WOS:000310796300001 ER PT J AU Martin, RL Prabhat Donofrio, DD Sethian, JA Haranczyk, M AF Martin, Richard L. Prabhat Donofrio, David D. Sethian, James A. Haranczyk, Maciej TI Accelerating analysis of void space in porous materials on multicore and GPU platforms SO INTERNATIONAL JOURNAL OF HIGH PERFORMANCE COMPUTING APPLICATIONS LA English DT Article DE code optimization; general purpose computation on GPUs; multicore programming; porous materials; screening; zeolites ID METAL-ORGANIC FRAMEWORKS; MOLECULAR SIMULATIONS; QUANTUM-CHEMISTRY; SHAPE SELECTIVITY; CARBON-DIOXIDE; ZEOLITES; ADSORPTION; IMPLEMENTATION; SEPARATION; DIFFUSION AB Developing computational tools that enable discovery of new materials for energy-related applications is a challenge. Crystalline porous materials are a promising class of materials that can be used for oil refinement, hydrogen or methane storage as well as carbon dioxide capture. Selecting optimal materials for these important applications requires analysis and screening of millions of potential candidates. Recently, we proposed an automatic approach based on the Fast Marching Method (FMM) for performing analysis of void space inside materials, a critical step preceding expensive molecular dynamics simulations. This breakthrough enables unsupervised, high-throughput characterization of large material databases. The algorithm has three steps: (1) calculation of the cost-grid which represents the structure and encodes the occupiable positions within the void space; (2) using FMM to segment out patches of the void space in the grid of (1), and find how they are connected to form either periodic channels or inaccessible pockets; and (3) generating blocking spheres that encapsulate the discovered inaccessible pockets and are used in proceeding molecular simulations. In this work, we expand upon our original approach through (A) replacement of the FMM-based approach with a more computationally efficient flood fill algorithm; and (B) parallelization of all steps in the algorithm, including a GPU implementation of the most computationally expensive step, the cost-grid generation. We report the acceleration achievable in each step and in the complete application, and discuss the implications for high-throughput material screening. C1 [Haranczyk, Maciej] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, Berkeley, CA 94720 USA. [Sethian, James A.] Univ Calif Berkeley, Dept Math, Berkeley, CA 94720 USA. RP Haranczyk, M (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, 1 Cyclotron Rd,MS 50F-1650, Berkeley, CA 94720 USA. EM mharanczyk@lbl.gov RI Martin, Richard/C-7129-2013; Haranczyk, Maciej/A-6380-2014 OI Martin, Richard/0000-0001-9858-2608; Haranczyk, Maciej/0000-0001-7146-9568 FU Office of Advanced Scientific Computing Research, Office of Science, of the U.S. Department of Energy through the Scientific Discovery through Advanced Computing (SciDAC) program's Visualization and Analytics Center for Enabling Technologies (VACET) [DE-AC02-05CH11231]; Applied Mathematical Science subprogram of the Office of Energy Research, U.S. Department of Energy [DE-AC03-76SF00098]; Computational Mathematics Program of the National Science Foundation FX This work was supported by the Director, Office of Advanced Scientific Computing Research, Office of Science, of the U.S. Department of Energy through the Scientific Discovery through Advanced Computing (SciDAC) program's Visualization and Analytics Center for Enabling Technologies (VACET) (Contract No. DE-AC02-05CH11231).; This work was also supported in part by the Applied Mathematical Science subprogram of the Office of Energy Research, U.S. Department of Energy (Contract Number DE-AC03-76SF00098), and by the Computational Mathematics Program of the National Science Foundation. NR 43 TC 10 Z9 10 U1 0 U2 21 PU SAGE PUBLICATIONS LTD PI LONDON PA 1 OLIVERS YARD, 55 CITY ROAD, LONDON EC1Y 1SP, ENGLAND SN 1094-3420 J9 INT J HIGH PERFORM C JI Int. J. High Perform. Comput. Appl. PD NOV PY 2012 VL 26 IS 4 SI SI BP 347 EP 357 DI 10.1177/1094342011431591 PG 11 WC Computer Science, Hardware & Architecture; Computer Science, Interdisciplinary Applications; Computer Science, Theory & Methods SC Computer Science GA 033KZ UT WOS:000310796300003 ER PT J AU Commer, M Maia, FRNC Newman, GA AF Commer, Michael Maia, Filipe R. N. C. Newman, Gregory A. TI Iterative Krylov solution methods for geophysical electromagnetic simulations on throughput-oriented processing units SO INTERNATIONAL JOURNAL OF HIGH PERFORMANCE COMPUTING APPLICATIONS LA English DT Article DE electromagnetic modeling; finite-difference methods; graphics processing unit; iterative Krylov methods; NVIDIA Compute Unified Device Architecture; parallel solutions ID BICONJUGATE GRADIENT-METHOD; LINEAR-SYSTEMS; QMR AB Many geo-scientific applications involve boundary value problems arising in simulating electrostatic and electromagnetic fields for geophysical prospecting and subsurface imaging of electrical resistivity. Modeling complex geological media with three-dimensional finite-difference grids gives rise to large sparse linear systems of equations. For such systems, we have implemented three common iterative Krylov solution methods on graphics processing units and compared their performance with parallel host-based versions. The benchmarks show that the device efficiency improves with increasing grid sizes. Limitations are currently given by the device memory resources. C1 [Commer, Michael; Newman, Gregory A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Maia, Filipe R. N. C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Natl Energy Res Sci Comp Ctr, Berkeley, CA 94720 USA. RP Commer, M (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. EM mcommer@lbl.gov RI Rocha Neves Couto Maia, Filipe/C-3146-2014; Commer, Michael/G-3350-2015 OI Rocha Neves Couto Maia, Filipe/0000-0002-2141-438X; Commer, Michael/0000-0003-0015-9217 FU Chevron Energy Technology Corporation; Petascale Initiative in Computational Science at NERSC; Office of Science, Advanced Scientific Computing Research, of the US Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Chevron Energy Technology Corporation and the Petascale Initiative in Computational Science at NERSC. It was also supported by the Director, Office of Science, Advanced Scientific Computing Research, of the US Department of Energy [Contract No. DE-AC02-05CH11231]. NR 18 TC 3 Z9 3 U1 0 U2 2 PU SAGE PUBLICATIONS LTD PI LONDON PA 1 OLIVERS YARD, 55 CITY ROAD, LONDON EC1Y 1SP, ENGLAND SN 1094-3420 J9 INT J HIGH PERFORM C JI Int. J. High Perform. Comput. Appl. PD NOV PY 2012 VL 26 IS 4 SI SI BP 378 EP 385 DI 10.1177/1094342011428145 PG 8 WC Computer Science, Hardware & Architecture; Computer Science, Interdisciplinary Applications; Computer Science, Theory & Methods SC Computer Science GA 033KZ UT WOS:000310796300006 ER PT J AU Joo, B Clark, MA AF Joo, Balint Clark, Mike A. TI Lattice QCD on GPU clusters, using the QUDA library and the Chroma software system SO INTERNATIONAL JOURNAL OF HIGH PERFORMANCE COMPUTING APPLICATIONS LA English DT Article DE Lattice QCD; GPU Computing; Chroma; QUDA; Nuclear Physics AB The QUDA library for optimized lattice quantum chromodynamics using GPUs, combined with a high-level application framework such as the Chroma software system, provides a powerful tool for computing quark propagators, a key step in current calculations of hadron spectroscopy, nuclear structure, and nuclear forces. In this contribution we discuss our experiences, including performance and strong scaling of the QUDA library and Chroma on the Edge Cluster at Lawrence Livermore National Laboratory and on various clusters at Jefferson Lab. We highlight some scientific successes and consider future directions for graphics processing units in lattice quantum chromodynamics calculations. C1 [Joo, Balint] Jefferson Lab, Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. [Clark, Mike A.] Harvard Smithsonian Ctr Astrophys, Cambridge, MA 02138 USA. RP Joo, B (reprint author), Jefferson Lab, Thomas Jefferson Natl Accelerator Facil, 12000 Jefferson Ave,Suite 3,MS 12B2,Room F217, Newport News, VA 23606 USA. EM bjoo@jlab.org FU U.S. DOE [DE-FC02-06ER41440, DE-FC02-06ER41449, DE-AC05-06OR23177]; NSF [OCI-1060067] FX Balint Joo gratefully acknowledges funding through U.S. DOE project grants DE-FC02-06ER41440 and DE-FC02-06ER41449 (USQCD SciDAC project) and DE-AC05-06OR23177 under which Jefferson Science Associates LLC manages and operates Jefferson Lab. Mike A Clark acknowledges funding under NSF grant OCI-1060067. NR 33 TC 2 Z9 2 U1 0 U2 6 PU SAGE PUBLICATIONS LTD PI LONDON PA 1 OLIVERS YARD, 55 CITY ROAD, LONDON EC1Y 1SP, ENGLAND SN 1094-3420 J9 INT J HIGH PERFORM C JI Int. J. High Perform. Comput. Appl. PD NOV PY 2012 VL 26 IS 4 SI SI BP 386 EP 398 DI 10.1177/1094342011429695 PG 13 WC Computer Science, Hardware & Architecture; Computer Science, Interdisciplinary Applications; Computer Science, Theory & Methods SC Computer Science GA 033KZ UT WOS:000310796300007 ER PT J AU Bethel, EW Howison, M AF Bethel, E. Wes Howison, Mark TI Multi-core and many-core shared-memory parallel raycasting volume rendering optimization and tuning SO INTERNATIONAL JOURNAL OF HIGH PERFORMANCE COMPUTING APPLICATIONS LA English DT Article DE parallel volume rendering; performance optimization; auto-tuning; multi-core CPU; many-core GPU AB Given the computing industry trend of increasing processing capacity by adding more cores to a chip, the focus of this work is tuning the performance of a staple visualization algorithm, raycasting volume rendering, for shared-memory parallelism on multi-core CPUs and many-core GPUs. Our approach is to vary tunable algorithmic settings, along with known algorithmic optimizations and two different memory layouts, and measure performance in terms of absolute runtime and L2 memory cache misses. Our results indicate there is a wide variation in runtime performance on all platforms, as much as 254% for the tunable parameters we test on multi-core CPUs and 265% on many-core GPUs, and the optimal configurations vary across platforms, often in a non-obvious way. For example, our results indicate the optimal configurations on the GPU occur at a crossover point between those that maintain good cache utilization and those that saturate computational throughput. This result is likely to be extremely difficult to predict with an empirical performance model for this particular algorithm because it has an unstructured memory access pattern that varies locally for individual rays and globally for the selected viewpoint. Our results also show that optimal parameters on modern architectures are markedly different from those in previous studies run on older architectures. In addition, given the dramatic performance variation across platforms for both optimal algorithm settings and performance results, there is a clear benefit for production visualization and analysis codes to adopt a strategy for performance optimization through auto-tuning. These benefits will likely become more pronounced in the future as the number of cores per chip and the cost of moving data through the memory hierarchy both increase. C1 [Bethel, E. Wes] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, Sci Visualizat Grp, Berkeley, CA 94720 USA. [Howison, Mark] Brown Univ, Ctr Computat & Visualizat, Providence, RI 02912 USA. RP Bethel, EW (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, Sci Visualizat Grp, 1 Cyclotron Rd,Mail Stop 50F, Berkeley, CA 94720 USA. EM ewbethel@lbl.gov OI Howison, Mark/0000-0002-0764-4090 FU Office of Science, Office and Advanced Scientific Computing Research, of the U.S. Department of Energy through the Scientific Discovery through Advanced Computing (SciDAC) program's Visualization and Analytics Center for Enabling Technologies (VACET) [DE-AC02-05CH11231]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231, DE-AC05-00OR22725]; National Energy Research Scientific Computing Center (NERSC); Brown University FX This work was supported by the Director, Office of Science, Office and Advanced Scientific Computing Research, of the U.S. Department of Energy (contract number DE-AC02-05CH11231) through the Scientific Discovery through Advanced Computing (SciDAC) program's Visualization and Analytics Center for Enabling Technologies (VACET). This work used resources of the National Center for Computational Sciences at Oak Ridge National Laboratory, which is supported by the Office of Science of the U.S. Department of Energy (contract number DE-AC05-00OR22725), and of the National Energy Research Scientific Computing Center (NERSC), which is supported by the Office of Science of the U.S. Department of Energy (contract number DE-AC02-05CH11231). This work was also supported by Brown University through the use of the facilities of its Center for Computation and Visualization. NR 39 TC 6 Z9 6 U1 1 U2 25 PU SAGE PUBLICATIONS LTD PI LONDON PA 1 OLIVERS YARD, 55 CITY ROAD, LONDON EC1Y 1SP, ENGLAND SN 1094-3420 J9 INT J HIGH PERFORM C JI Int. J. High Perform. Comput. Appl. PD NOV PY 2012 VL 26 IS 4 SI SI BP 399 EP 412 DI 10.1177/1094342012440466 PG 14 WC Computer Science, Hardware & Architecture; Computer Science, Interdisciplinary Applications; Computer Science, Theory & Methods SC Computer Science GA 033KZ UT WOS:000310796300008 ER PT J AU Halappanavar, M Feo, J Villa, O Tumeo, A Pothen, A AF Halappanavar, Mahantesh Feo, John Villa, Oreste Tumeo, Antonino Pothen, Alex TI Approximate weighted matching on emerging manycore and multithreaded architectures SO INTERNATIONAL JOURNAL OF HIGH PERFORMANCE COMPUTING APPLICATIONS LA English DT Article DE approximation; dataflow; GPU; graph algorithms; manycore; matching; multicore; weighted matching ID GRAPH ALGORITHMS; PERFORMANCE; CUDA AB Graph matching is a prototypical combinatorial problem with many applications in high-performance scientific computing. Optimal algorithms for computing matchings are challenging to parallelize. Approximation algorithms are amenable to parallelization and are therefore important to compute matchings for large-scale problems. Approximation algorithms also generate nearly optimal solutions that are sufficient for many applications. In this paper we present multithreaded algorithms for computing half-approximate weighted matching on state-of-the-art multicore (Intel Nehalem and AMD Magny-Cours), manycore (Nvidia Tesla and Nvidia Fermi), and massively multithreaded (Cray XMT) platforms. We provide two implementations: the first uses shared work queues and is suited for all platforms; and the second implementation, based on dataflow principles, exploits special features available on the Cray XMT. Using a carefully chosen dataset that exhibits characteristics from a wide range of applications, we show scalable performance across different platforms. In particular, for one instance of the input, an R-MAT graph (RMAT-G), we show speedups of about 32 on 48 cores of an AMD Magny-Cours, 7 on 8 cores of Intel Nehalem, 3 on Nvidia Tesla and 10 on Nvidia Fermi relative to one core of Intel Nehalem, and 60 on 128 processors of Cray XMT. We demonstrate strong as well as weak scaling for graphs with up to a billion edges using up to 12,800 threads. We avoid excessive fine-tuning for each platform and retain the basic structure of the algorithm uniformly across platforms. An exception is the dataflow algorithm designed specifically for the Cray XMT. To the best of the authors' knowledge, this is the first such large-scale study of the half-approximate weighted matching problem on multithreaded platforms. Driven by the critical enabling role of combinatorial algorithms such as matching in scientific computing and the emergence of informatics applications, there is a growing demand to support irregular computations on current and future computing platforms. In this context, we evaluate the capability of emerging multithreaded platforms to tolerate latency induced by irregular memory access patterns, and to support fine-grained parallelism via light-weight synchronization mechanisms. By contrasting the architectural features of these platforms against the Cray XMT, which is specifically designed to support irregular memory-intensive applications, we delineate the impact of these choices on performance. C1 [Halappanavar, Mahantesh] Pacific NW Natl Lab, Computat Sci & Math Div, Richland, WA 99352 USA. [Pothen, Alex] Purdue Univ, W Lafayette, IN 47907 USA. RP Halappanavar, M (reprint author), Pacific NW Natl Lab, Computat Sci & Math Div, 902 Battelle Blvd,POB 999,MSIN J4-30, Richland, WA 99352 USA. EM mahantesh.halappanavar@pnl.gov RI Tumeo, Antonino/L-3106-2016; OI Pothen, Alex/0000-0002-3421-3325 FU Center for Adaptive Super Computing Software - MultiThreaded Architectures (CASS-MT) at the U.S. Department of Energy's Pacific Northwest National Laboratory; Battelle Memorial Institute [DE-ACO6-76RL01830]; U.S. Department of Energy through the CSCAPES Institute [DE-FC02-08ER25864, DE-FC02-06ER2775] FX This work was supported by the Center for Adaptive Super Computing Software - MultiThreaded Architectures (CASS-MT) at the U.S. Department of Energy's Pacific Northwest National Laboratory. PNNL is operated by the Battelle Memorial Institute (contract number DE-ACO6-76RL01830). Additional funding for this project was provided by the U.S. Department of Energy through the CSCAPES Institute (grant numbers DE-FC02-08ER25864 and DE-FC02-06ER2775). NR 33 TC 12 Z9 12 U1 0 U2 3 PU SAGE PUBLICATIONS LTD PI LONDON PA 1 OLIVERS YARD, 55 CITY ROAD, LONDON EC1Y 1SP, ENGLAND SN 1094-3420 J9 INT J HIGH PERFORM C JI Int. J. High Perform. Comput. Appl. PD NOV PY 2012 VL 26 IS 4 SI SI BP 413 EP 430 DI 10.1177/1094342012452893 PG 18 WC Computer Science, Hardware & Architecture; Computer Science, Interdisciplinary Applications; Computer Science, Theory & Methods SC Computer Science GA 033KZ UT WOS:000310796300009 ER PT J AU Oset, E Ramos, A Garzon, EJ Molina, R Tolos, L Xiao, CW Wu, JJ Zou, BS AF Oset, E. Ramos, A. Garzon, E. J. Molina, R. Tolos, L. Xiao, C. W. Wu, J. J. Zou, B. S. TI INTERACTION OF VECTOR MESONS WITH BARYONS AND NUCLEI SO INTERNATIONAL JOURNAL OF MODERN PHYSICS E-NUCLEAR PHYSICS LA English DT Review DE Vector-baryon interaction; vectors in medium; J/psi suppression in nuclei ID HEAVY-ION COLLISIONS; CHIRAL DYNAMICS; RHO-MESON; HADRON PROPERTIES; MATTER; RESONANCE; PHOTOPRODUCTION; LAMBDA(1405); LAGRANGIANS; SYMMETRY AB After some short introductory remarks on particular issues on the vector mesons in nuclei, in this paper, we present a short review of recent developments concerning the interaction of vector mesons with baryons and with nuclei from a modern perspective using the local hidden gauge formalism for the interaction of vector mesons. We present results for the vector-baryon interaction and in particular for the resonances which appear as composite states, dynamically generated from the interaction of vector mesons with baryons, taking also the mixing of these states with pseudoscalars and baryons into account. We then venture into the charm sector, reporting on hidden charm baryon states around 4400 MeV, generated from the interaction of vector mesons and baryons with charm, which have a strong repercussion on the properties of the J/Psi N interaction. We also address the interaction of K* with nuclei and make suggestions to measure the predicted huge width in the medium by means of transparency ratio. The formalism is extended to study the phenomenon of J/psi suppression in nuclei via J/psi photo-production reactions. C1 [Oset, E.; Garzon, E. J.; Xiao, C. W.] Univ Valencia, CSIC, Inst Invest Paterna, Dept Fis Teor, Valencia 46071, Spain. [Oset, E.; Garzon, E. J.; Xiao, C. W.] Univ Valencia, CSIC, Inst Invest Paterna, IFIC,Ctr Mixto, Valencia 46071, Spain. [Ramos, A.] Univ Barcelona, Dept Estruct & Constituents Mat, Barcelona, Spain. [Molina, R.] RCNP, Ibaraki 5670047, Japan. [Tolos, L.] CSIC, Inst Ciencias Espacio IEEC, Fac Ciencias, E-08193 Bellaterra, Barcelona, Spain. [Tolos, L.] Goethe Univ Frankfurt, FIAS, D-60438 Frankfurt, Germany. [Wu, J. J.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Zou, B. S.] Chinese Acad Sci, Inst High Energy Phys, Beijing 100049, Peoples R China. [Zou, B. S.] Chinese Acad Sci, Theoret Phys Ctr Sci Facilit, Beijing 100049, Peoples R China. RP Oset, E (reprint author), Univ Valencia, CSIC, Inst Invest Paterna, Dept Fis Teor, Aptdo 22085, Valencia 46071, Spain. EM oset@ific.uv.es RI Ramos, Angels/L-3043-2014; Tolos, Laura/F-2515-2016; OI Ramos, Angels/0000-0002-0882-1570; Tolos, Laura/0000-0003-2304-7496; Molina, Raquel/0000-0001-9427-240X FU DGICYT [FIS2011-28853-C02-01, FIS2011-24154]; Generalitat Valenciana in the program Prometeo [2009/090]; Generalitat de Catalunya [2009SGR-1289]; Ramon y Cajal Research Programme; FP7-PEOPLE-2011-CIG [PCIG09-GA-2011-291679]; European Community-Research Infrastructure Integrating Activity Study of Strongly Interacting Matter under the Seventh Framework Programme of EU [283286] FX This work is partly supported by DGICYT contract numbers FIS2011-28853-C02-01, FIS2011-24154, the Generalitat Valenciana in the program Prometeo, 2009/090 and Grant No. 2009SGR-1289 from Generalitat de Catalunya. LT acknowledges support from Ramon y Cajal Research Programme, and from FP7-PEOPLE-2011-CIG under contract PCIG09-GA-2011-291679. We acknowledge the support of the European Community-Research Infrastructure Integrating Activity Study of Strongly Interacting Matter (acronym HadronPhysics3, Grant Agreement No. 283286) under the Seventh Framework Programme of EU. NR 86 TC 33 Z9 33 U1 0 U2 3 PU WORLD SCIENTIFIC PUBL CO PTE LTD PI SINGAPORE PA 5 TOH TUCK LINK, SINGAPORE 596224, SINGAPORE SN 0218-3013 EI 1793-6608 J9 INT J MOD PHYS E JI Int. J. Mod. Phys. E-Nucl. Phys. PD NOV PY 2012 VL 21 IS 11 AR 1230011 DI 10.1142/S0218301312300111 PG 18 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA 034FM UT WOS:000310855800002 ER PT J AU Wen, ZW Yang, C Liu, X Marchesini, S AF Wen, Zaiwen Yang, Chao Liu, Xin Marchesini, Stefano TI Alternating direction methods for classical and ptychographic phase retrieval SO INVERSE PROBLEMS LA English DT Article ID ALGORITHM; OPTIMIZATION AB In this paper, we show how the augmented Lagrangian alternating direction method (ADM) can be used to solve both the classical and ptychographic phase retrieval problems. We point out the connection between ADM and projection algorithms such as the hybrid input-output algorithm, and compare its performance against standard algorithms for phase retrieval on a number of test images. Our computational experiments show that ADM appears to be less sensitive to the choice of relaxation parameters, and it usually outperforms the existing techniques for both the classical and ptychographic phase retrieval problems. C1 [Wen, Zaiwen] Shanghai Jiao Tong Univ, Dept Math, MOE LSC, Shanghai 200240, Peoples R China. [Wen, Zaiwen] Shanghai Jiao Tong Univ, Inst Nat Sci, Shanghai 200240, Peoples R China. [Yang, Chao] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, Berkeley, CA 94720 USA. [Liu, Xin] Chinese Acad Sci, State Key Lab Sci & Engn Comp, Acad Math & Syst Sci, Beijing 100080, Peoples R China. [Marchesini, Stefano] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Wen, ZW (reprint author), Shanghai Jiao Tong Univ, Dept Math, MOE LSC, Shanghai 200240, Peoples R China. EM zw2109@sjtu.edu.cn; cyang@lbl.gov; liuxin@lsec.cc.ac.cn; smarchesini@lbl.gov FU NSFC [11101274, 11101409, 10831006]; research fund for the Doctoral Program of Higher Education of China; Shanghai Pujiang Program [12PJ1404800]; Laboratory Directed Research and Development Program of Lawrence Berkeley National Laboratory under the US Department of Energy [DE-AC02-05CH11231]; National Center for Mathematics and Interdisciplinary Sciences, CAS FX The work of ZW is supported in part by NSFC grant 11101274, a research fund for the Doctoral Program of Higher Education of China and Shanghai Pujiang Program 12PJ1404800. The work of CY and SM is supported by the Laboratory Directed Research and Development Program of Lawrence Berkeley National Laboratory under the US Department of Energy contract number DE-AC02-05CH11231. The work of XL is supported in part by NSFC grants 11101409 and 10831006, and the National Center for Mathematics and Interdisciplinary Sciences, CAS. NR 26 TC 16 Z9 16 U1 0 U2 13 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0266-5611 J9 INVERSE PROBL JI Inverse Probl. PD NOV PY 2012 VL 28 IS 11 AR 115010 DI 10.1088/0266-5611/28/11/115010 PG 18 WC Mathematics, Applied; Physics, Mathematical SC Mathematics; Physics GA 030MK UT WOS:000310574600010 ER PT J AU Pester, M Brambilla, E Alazard, D Rattei, T Weinmaier, T Han, J Lucas, S Lapidus, A Cheng, JF Goodwin, L Pitluck, S Peters, L Ovchinnikova, G Teshima, H Detter, JC Han, CS Tapia, R Land, ML Hauser, L Kyrpides, NC Ivanova, NN Pagani, I Huntmann, M Wei, CL Davenport, KW Daligault, H Chain, PSG Chen, A Mavromatis, K Markowitz, V Szeto, E Mikhailova, N Pati, A Wagner, M Woyke, T Ollivier, B Klenk, HP Spring, S Loy, A AF Pester, Michael Brambilla, Evelyne Alazard, Didier Rattei, Thomas Weinmaier, Thomas Han, James Lucas, Susan Lapidus, Alla Cheng, Jan-Fang Goodwin, Lynne Pitluck, Sam Peters, Lin Ovchinnikova, Galina Teshima, Hazuki Detter, John C. Han, Cliff S. Tapia, Roxanne Land, Miriam L. Hauser, Loren Kyrpides, Nikos C. Ivanova, Natalia N. Pagani, Ioanna Huntmann, Marcel Wei, Chia-Lin Davenport, Karen W. Daligault, Hajnalka Chain, Patrick S. G. Chen, Amy Mavromatis, Konstantinos Markowitz, Victor Szeto, Ernest Mikhailova, Natalia Pati, Amrita Wagner, Michael Woyke, Tanja Ollivier, Bernard Klenk, Hans-Peter Spring, Stefan Loy, Alexander TI Complete Genome Sequences of Desulfosporosinus orientis DSM765(T), Desulfosporosinus youngiae DSM17734(T), Desulfosporosinus meridiei DSM13257(T), and Desulfosporosinus acidiphilus DSM22704(T) SO JOURNAL OF BACTERIOLOGY LA English DT Article ID SULFATE-REDUCING BACTERIUM; ACID-MINE DRAINAGE; SP-NOV.; REDUCTION; WATER; LAKE AB Desulfosporosinus species are sulfate-reducing bacteria belonging to the Firmicutes. Their genomes will give insights into the genetic repertoire and evolution of sulfate reducers typically thriving in terrestrial environments and able to degrade toluene (Desulfosporosinus youngiae), to reduce Fe(III) (Desulfosporosinus meridiei, Desulfosporosinus orientis), and to grow under acidic conditions (Desulfosporosinus acidiphilus). C1 [Pester, Michael; Wagner, Michael; Loy, Alexander] Univ Vienna, Fac Life Sci, Dept Microbial Ecol, Vienna, Austria. [Brambilla, Evelyne; Klenk, Hans-Peter; Spring, Stefan] Deutsch Sammlung Mikroorganism Zellkultur GmbH, Leibniz Inst, Braunschweig, Germany. [Alazard, Didier; Ollivier, Bernard] Aix Marseille Univ, CNRS, MIO, UMR IRD 235,UMR 7294,Equipe MEB,ESIL, Marseille, France. [Rattei, Thomas; Weinmaier, Thomas] Univ Vienna, Fac Life Sci, Dept Computat Syst Biol, Vienna, Austria. [Han, James; Lapidus, Alla; Cheng, Jan-Fang; Pitluck, Sam; Peters, Lin; Ovchinnikova, Galina; Detter, John C.; Han, Cliff S.; Tapia, Roxanne; Land, Miriam L.; Hauser, Loren; Kyrpides, Nikos C.; Ivanova, Natalia N.; Pagani, Ioanna; Huntmann, Marcel; Chain, Patrick S. G.; Chen, Amy; Mavromatis, Konstantinos; Szeto, Ernest; Mikhailova, Natalia; Pati, Amrita; Woyke, Tanja] US DOE, Joint Genome Inst, Walnut Creek, CA USA. [Lucas, Susan; Goodwin, Lynne; Teshima, Hazuki; Detter, John C.; Han, Cliff S.; Tapia, Roxanne; Wei, Chia-Lin; Davenport, Karen W.; Daligault, Hajnalka; Markowitz, Victor] Los Alamos Natl Lab, Joint Genome Inst, Biosci Div Genome Sci, Los Alamos, NM USA. [Land, Miriam L.; Hauser, Loren] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN USA. RP Pester, M (reprint author), Univ Vienna, Fac Life Sci, Dept Microbial Ecol, Vienna, Austria. EM pester@microbial-ecology.net RI Kyrpides, Nikos/A-6305-2014; Loy, Alexander/A-8182-2008; Pester, Michael/A-3870-2013; Pagani, Ioanna/E-7390-2012; chain, patrick/B-9777-2013; Lapidus, Alla/I-4348-2013; Land, Miriam/A-6200-2011; Spring, Stefan/N-6933-2013; Wagner, Michael/A-7801-2011; Rattei, Thomas/F-1366-2011; Ollivier, Bernard/I-6150-2016 OI Kyrpides, Nikos/0000-0002-6131-0462; Loy, Alexander/0000-0001-8923-5882; Pester, Michael/0000-0001-6296-4145; Lapidus, Alla/0000-0003-0427-8731; Weinmaier, Thomas/0000-0002-9552-3220; Land, Miriam/0000-0001-7102-0031; Spring, Stefan/0000-0001-6247-0938; Wagner, Michael/0000-0002-9778-7684; Rattei, Thomas/0000-0002-0592-7791; FU Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; Austrian Science Fund [P23117-B17, P20185-B17] FX The work conducted by the U.S. Department of Energy Joint Genome Institute is supported by the Office of Science of the U.S. Department of Energy under contract no. DE-AC02-05CH11231. This research was further financially supported by the Austrian Science Fund (P23117-B17 to M. Pester; P20185-B17 to A. Loy). NR 24 TC 19 Z9 19 U1 2 U2 20 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 0021-9193 J9 J BACTERIOL JI J. Bacteriol. PD NOV PY 2012 VL 194 IS 22 BP 6300 EP 6301 DI 10.1128/JB.01392-12 PG 2 WC Microbiology SC Microbiology GA 030SB UT WOS:000310589300032 PM 23105050 ER PT J AU Trimble, WL Phung, LT Meyer, F Silver, S Gilbert, JA AF Trimble, William L. Phung, Le T. Meyer, Folker Silver, Simon Gilbert, Jack A. TI Draft Genome Sequence of Achromobacter piechaudii Strain HLE SO JOURNAL OF BACTERIOLOGY LA English DT Article ID ALCALIGENES-FAECALIS; ARSENITE; OXIDATION AB Achromobacter piechaudii strain HLE is a betaproteobacterium (previously known as Alcaligenes faecalis) that was an early isolate with arsenite oxidase activity. This draft genome of 6.89 Mb is the second available genome for this species in the opportunistic pathogen Alcaligenaceae family. C1 [Phung, Le T.; Silver, Simon] Univ Illinois, Dept Microbiol & Immunol, Chicago, IL 60680 USA. [Trimble, William L.; Meyer, Folker; Gilbert, Jack A.] Argonne Natl Lab, Inst Genom & Syst Biol, Argonne, IL 60439 USA. [Gilbert, Jack A.] Univ Chicago, Dept Ecol & Evolut, Chicago, IL 60637 USA. RP Silver, S (reprint author), Univ Illinois, Dept Microbiol & Immunol, Chicago, IL 60680 USA. EM simon@uic.edu; gilbertjack@anl.gov OI Trimble, William L./0000-0001-7029-2676; Meyer, Folker/0000-0003-1112-2284; Silver, Simon/0000-0002-5692-3125 FU U.S. Department of Energy FX This work was supported by funds from the U.S. Department of Energy. NR 10 TC 6 Z9 6 U1 1 U2 3 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 0021-9193 J9 J BACTERIOL JI J. Bacteriol. PD NOV PY 2012 VL 194 IS 22 BP 6355 EP 6355 DI 10.1128/JB.01660-12 PG 1 WC Microbiology SC Microbiology GA 030SB UT WOS:000310589300067 PM 23105084 ER PT J AU Kail, BW Link, DD Morreale, BD AF Kail, Brian W. Link, Dirk D. Morreale, Bryan D. TI Determination of Free Fatty Acids and Triglycerides by Gas Chromatography Using Selective Esterification Reactions SO JOURNAL OF CHROMATOGRAPHIC SCIENCE LA English DT Article ID TRANSESTERIFICATION; EXTRACTION; BIODIESEL AB A method for selectively determining both free fatty acids (FFA) and triacylglycerides (TAGs) in biological oils was investigated and optimized using gas chromatography after esterification of the target species to their corresponding fatty acid methyl esters (FAMEs). The method used acid catalyzed esterification in methanolic solutions under conditions of varying severity to achieve complete conversion of more reactive FFAs while preserving the concentration of TAGs. Complete conversion of both free acids and glycerides to corresponding FAMEs was found to require more rigorous reaction conditions involving heating to 120 degrees C for up to 2 h. Method validation was provided using gas chromatography-flame ionization detection, gas chromatography-mass spectrometry, and liquid chromatography-mass spectrometry. The method improves on existing methods because it allows the total esterified lipid to be broken down by FAMEs contributed by FFA compared to FAMEs from both FFA and TAGs. Single and mixed-component solutions of pure fatty acids and triglycerides, as well as a sesame oil sample to simulate a complex biological oil, were used to optimize the methodologies. Key parameters that were investigated included: HCl-to-oil ratio, temperature and reaction time. Pure free fatty acids were found to esterify under reasonably mild conditions (10 min at 50 degrees C with a 2.1:1 HCl to fatty acid ratio) with 97.6 +/- 2.3% recovery as FAMEs, while triglycerides were largely unaffected under these reaction conditions. The optimized protocol demonstrated that it is possible to use esterification reactions to selectively determine the free acid content, total lipid content, and hence, glyceride content in biological oils. This protocol also allows gas chromatography analysis of FAMEs as a more ideal analyte than glyceride species in their native state. C1 [Kail, Brian W.; Link, Dirk D.; Morreale, Bryan D.] US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. [Kail, Brian W.] URS, South Pk, PA 15219 USA. RP Kail, BW (reprint author), US DOE, Natl Energy Technol Lab, POB 10940, Pittsburgh, PA 15236 USA. EM brian.kail@ur.netl.doe.gov NR 15 TC 0 Z9 0 U1 5 U2 58 PU OXFORD UNIV PRESS INC PI CARY PA JOURNALS DEPT, 2001 EVANS RD, CARY, NC 27513 USA SN 0021-9665 J9 J CHROMATOGR SCI JI J. Chromatogr. Sci. PD NOV-DEC PY 2012 VL 50 IS 10 BP 934 EP 939 DI 10.1093/chromsci/bms093 PG 6 WC Biochemical Research Methods; Chemistry, Analytical SC Biochemistry & Molecular Biology; Chemistry GA 033RU UT WOS:000310819400013 PM 22695884 ER PT J AU Kiener, D Minor, AM Anderoglu, O Wang, YQ Maloy, SA Hosemann, P AF Kiener, Daniel Minor, Andrew M. Anderoglu, Osman Wang, Yongqiang Maloy, Stuart A. Hosemann, Peter TI Application of small-scale testing for investigation of ion-beam-irradiated materials SO JOURNAL OF MATERIALS RESEARCH LA English DT Article ID TRANSMISSION ELECTRON-MICROSCOPY; SENSING INDENTATION EXPERIMENTS; STACKING-FAULT TETRAHEDRON; PLASTICITY FINITE-ELEMENT; CRYSTAL PLASTICITY; MECHANICAL-PROPERTIES; NEUTRON-IRRADIATION; SINGLE-CRYSTALS; MICROPILLAR COMPRESSION; RADIATION-DAMAGE AB Small-scale testing techniques such as nanoindentation and micro-/nanocompression are promising methods for addressing mechanical properties of ion-beam-irradiated materials. We performed different proton irradiations and critically evaluated the results obtained from nanoindentation and pillar compression, both performed parallel and perpendicular to the irradiation direction. Experiments parallel to beam direction suffer from variation of material properties with penetration depth. This is improved by cross-sectional experiments, thereby probing the effect of different doses along the beam penetration depth on mechanical properties. Finally, we demonstrate that, compared with nanoindentation, miniaturized uniaxial compression experiments offer a more reliable and straightforward interpretation of the mechanical data, as they impose a nominally uniaxial stress on a well-defined volume at a specific position. Moreover, the exposed pillar geometry is not influenced by surface contamination and enables in situ observation of the governing mechanical processes, which is typically not possible during indentation experiments in a half-space geometry. C1 [Kiener, Daniel] Univ Leoben, Dept Mat Phys, A-8700 Leoben, Austria. [Kiener, Daniel; Minor, Andrew M.] Univ Calif Berkeley, Dept Mat Sci, Berkeley, CA 94720 USA. [Minor, Andrew M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Natl Ctr Electron Microscopy, Berkeley, CA 94720 USA. [Anderoglu, Osman; Wang, Yongqiang; Maloy, Stuart A.] Los Alamos Natl Lab, Mat Sci & Technol Div, Los Alamos, NM 87545 USA. [Hosemann, Peter] Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA. RP Kiener, D (reprint author), Univ Leoben, Dept Mat Phys, A-8700 Leoben, Austria. EM daniel.kiener@unileoben.ac.at RI Lujan Center, LANL/G-4896-2012; Maloy, Stuart/A-8672-2009; Kiener, Daniel/B-2202-2008; OI Maloy, Stuart/0000-0001-8037-1319; Kiener, Daniel/0000-0003-3715-3986; Hosemann, Peter/0000-0003-2281-2213 FU Center for Integrated Nanotechnologies (CINT), a DOE nanoscience center; Berkeley nuclear research center (BNRC); NRC faculty development grant [NRC-38-09-948]; Austrian Science Fund (FWF) [J2834-N20]; U.S. Department of Energy [DE-AC02-05CH11231] FX Ion irradiation and nanoindentation work was partially supported by Center for Integrated Nanotechnologies (CINT), a DOE nanoscience center jointly operated by Los Alamos and Sandia National Laboratories. Funding was provided partially by the Berkeley nuclear research center (BNRC), established by the University of California Office of the President and the UC-National Laboratory Fee Research Program as well as by the NRC faculty development grant, NRC-38-09-948. DK gratefully acknowledges financial support of the Austrian Science Fund (FWF) through the project J2834-N20. The in situ TEM experiments were performed at the National Center for Electron Microscopy, Lawrence Berkeley National Laboratory, which is supported by the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 81 TC 15 Z9 15 U1 8 U2 77 PU CAMBRIDGE UNIV PRESS PI NEW YORK PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA SN 0884-2914 J9 J MATER RES JI J. Mater. Res. PD NOV PY 2012 VL 27 IS 21 BP 2724 EP 2736 DI 10.1557/jmr.2012.303 PG 13 WC Materials Science, Multidisciplinary SC Materials Science GA 032HM UT WOS:000310706100004 ER PT J AU Engtrakul, C Curtis, CJ Ellis, JE Gedvilas, LM Blackburn, JL Simpson, LJ Jones, KM Parilla, PA Dillon, AC Heben, MJ Gennett, T AF Engtrakul, Chaiwat Curtis, Calvin J. Ellis, Jamie E. Gedvilas, Lynn M. Blackburn, Jeffrey L. Simpson, Lin J. Jones, Kim M. Parilla, Philip A. Dillon, Anne C. Heben, Michael J. Gennett, Thomas TI Reactions and reversible hydrogenation of single-walled carbon nanotube anions SO JOURNAL OF MATERIALS RESEARCH LA English DT Article ID RAMAN-SPECTROSCOPY; ATOMIC-HYDROGEN; CHARGE-TRANSFER; GLOW-DISCHARGE; FUNCTIONALIZATION; GRAPHITE; SODIUM; METAL; SALTS; WATER AB Single-walled carbon nanotube (SWNT) radical anions will react with tetrahydrofuran and generate ethylene, enolates, and a partially hydrogenated nanotube backbone. The experimental evidence suggests that there are sp(3) C-H binding interactions. The total gravimetric content of hydrogen on a sample averages from 3.5% to 3.9% w/w, about four times the total amount observed for nanotubes hydrogenated via traditional Birch reduction reactions. Furthermore, the hydrogen desorbs at temperatures up to 400 degrees C less than those observed for the hydrogenated SWNTs formed after the Birch reduction. Finally, the first room temperature electron spin resonance spectrum of a nanotube radical ion is also reported. C1 [Engtrakul, Chaiwat; Curtis, Calvin J.; Ellis, Jamie E.; Gedvilas, Lynn M.; Blackburn, Jeffrey L.; Simpson, Lin J.; Jones, Kim M.; Parilla, Philip A.; Dillon, Anne C.; Heben, Michael J.; Gennett, Thomas] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Gennett, T (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM thomas.gennett@nrel.gov RI Engtrakul, Chaiwat/H-5634-2011 FU U.S. Department of Energy's Office of Energy Efficiency and Renewable Energy within the Center of Excellence on Hydrogen Sorption Materials, DOE's National Hydrogen Storage Grand Challenge; Office of Science, Basic Energy Sciences, Materials Science and Engineering [DE-AC36-99GO10337] FX Funding for this effort was provided by the U.S. Department of Energy's Office of Energy Efficiency and Renewable Energy within the Center of Excellence on Hydrogen Sorption Materials as part of DOE's National Hydrogen Storage Grand Challenge and by the Office of Science, Basic Energy Sciences, Materials Science and Engineering under subcontract DE-AC36-99GO10337 to NREL. NR 36 TC 2 Z9 2 U1 0 U2 24 PU CAMBRIDGE UNIV PRESS PI NEW YORK PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA SN 0884-2914 J9 J MATER RES JI J. Mater. Res. PD NOV PY 2012 VL 27 IS 21 BP 2806 EP 2811 DI 10.1557/jmr.2012.298 PG 6 WC Materials Science, Multidisciplinary SC Materials Science GA 032HM UT WOS:000310706100013 ER PT J AU Elvington, MC Tosten, M Taylor-Pashow, KML Hobbs, DT AF Elvington, M. C. Tosten, M. Taylor-Pashow, K. M. L. Hobbs, D. T. TI Synthesis and characterization of nanosize sodium titanates SO JOURNAL OF NANOPARTICLE RESEARCH LA English DT Article DE Sol-gel; Surfactant; Ion exchange; Hydrogen peroxide ID NUCLEAR-WASTE SOLUTIONS; MONOSODIUM TITANATE; ACTINIDE SEPARATIONS; STRONTIUM; PEROXOTITANATE; PHOTOCATALYSTS; SORPTION; REMOVAL AB This paper describes the synthesis and peroxide-modification of nanosize monosodium titanate (nMST). The synthesis method was derived from a sol-gel process used to produce micron-sized monosodium titanate (MST). Key modifications to this process include altering reagent concentrations, omitting a particle seed step, and introducing a non-ionic surfactant to facilitate control of particle formation and growth. The nMST material exhibits spherical-shaped particle morphology with a monodisperse distribution of particle diameters in the range from 100 to 150 nm. The BET surface area and isoelectric point of then MST measured 285 m(2) g(-1) and 3.34 pH units, respectively, which is more than an order of magnitude higher in surface area and a pH unit lower than that measured for the microsize MST. The nMST material serves as an effective ion exchanger under both weakly acidic and strongly alkaline conditions and was converted to a peroxotitanate form by reaction with hydrogen peroxide. C1 [Elvington, M. C.; Tosten, M.; Taylor-Pashow, K. M. L.; Hobbs, D. T.] Savannah River Natl Lab, Aiken, SC 29808 USA. RP Hobbs, DT (reprint author), Savannah River Natl Lab, Aiken, SC 29808 USA. EM david.hobbs@srnl.doe.gov FU Laboratory Directed Research and Development program at the Savannah River National Laboratory (SRNL); University of Washington; National Institute of Health [1R01DE021373-01]; Department of Energy [DE-AC09-08SR22470] FX The authors thank the Laboratory Directed Research and Development program at the Savannah River National Laboratory (SRNL) for funding. We thank Dr. Fernando Fondeur for collection and interpretation of the FT-IR spectra and Dr. John Seaman of the Savannah River Ecology Laboratory for the use of the DLS instrument for particle size measurements. We also thank the Dr. Daniel Chan of the University of Washington and the National Institute of Health (Grant #1R01DE021373-01), for funding experiments investigating the ion exchange reactions with Au(III). The Savannah River National Laboratory is operated by Savannah River Nuclear Solutions, LLC for the Department of Energy under contract DE-AC09-08SR22470. NR 31 TC 4 Z9 4 U1 3 U2 33 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 1388-0764 J9 J NANOPART RES JI J. Nanopart. Res. PD NOV PY 2012 VL 14 IS 11 AR 1114 DI 10.1007/s11051-012-1114-z PG 12 WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 030ZG UT WOS:000310608100030 ER PT J AU Jonah, EO Britton, DT Beaucage, P Rai, DK Beaucage, G Magunje, B Ilavsky, J Scriba, MR Harting, M AF Jonah, E. O. Britton, D. T. Beaucage, P. Rai, D. K. Beaucage, G. Magunje, B. Ilavsky, J. Scriba, M. R. Haerting, M. TI Topological investigation of electronic silicon nanoparticulate aggregates using ultra-small-angle X-ray scattering SO JOURNAL OF NANOPARTICLE RESEARCH LA English DT Article DE Ultra-small-angle X-ray scattering; Semiconductor nanocomposites; Network structures; Fractals; Printed electronics ID CONTROLLED CLUSTER FORMATION; FIELD-EFFECT TRANSISTORS; COMPUTER-SIMULATION; PERCOLATION; RESOLUTION; DEVICES AB The network topology of two types of silicon nanoparticles, produced by high energy milling and pyrolysis of silane, in layers deposited from inks on permeable and impermeable substrates has been quantitatively characterized using ultra-small-angle X-ray scattering, supported by scanning electron microscopy observations. The milled particles with a highly polydisperse size distribution form agglomerates, which in turn cluster to form larger aggregates with a very high degree of aggregation. Smaller nanoparticles with less polydisperse size distribution synthesized by thermal catalytic pyrolysis of silane form small open clusters. The Sauter mean diameters of the primary particles of the two types of nanoparticles were obtained from USAXS particle volume to surface ratio, with values of similar to 41 and similar to 21 nm obtained for the high energy milled and pyrolysis samples, respectively. Assuming a log-normal distribution of the particles, the geometric standard deviation of the particles was calculated to be similar to 1.48 for all the samples, using parameters derived from the unified fit to the USAXS data. The flow properties of the inks and substrate combination lead to quantitative changes in the mean particle separation, with slowly curing systems with good capillary flow resulting in denser networks with smaller aggregates and better contact between particles. C1 [Jonah, E. O.; Britton, D. T.; Magunje, B.; Scriba, M. R.; Haerting, M.] Univ Cape Town, Dept Phys, NanoSci Innovat Ctr, ZA-7701 Rondebosch, South Africa. [Beaucage, P.; Rai, D. K.; Beaucage, G.] Univ Cincinnati, Dept Chem & Mat Engn, Cincinnati, OH 45221 USA. [Ilavsky, J.] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. [Scriba, M. R.] CSIR, Natl Ctr Nanostruct Mat, ZA-0001 Pretoria, South Africa. RP Jonah, EO (reprint author), Univ Cape Town, Dept Phys, NanoSci Innovat Ctr, ZA-7701 Rondebosch, South Africa. EM emmanuel.jonah@uct.ac.za RI Ilavsky, Jan/D-4521-2013; USAXS, APS/D-4198-2013; OI Ilavsky, Jan/0000-0003-1982-8900; Rai, Durgesh/0000-0001-7257-7210 FU NanoPower Africa Project; United States Agency for International Development (USAID) through the Higher Education for Development (HED) office; LyondellBasell, LP; National Science Foundation [0626063]; PG Corporation; US Airforce Office of Scientific Research; University of Cape Town Vice Chancellor's Strategic Fund; South African National Research Foundation (NRF) [FA20064160004]; South African Department of Science and Technology through its business unit the Innovation Fund under Technology Advancement Project [T50055]; National Science Foundation/Department of Energy [NSF/CHE-0822838]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work was in part supported by the NanoPower Africa Project funded by United States Agency for International Development (USAID) through the Higher Education for Development (HED) office. The contents are the responsibility of the authors and do not necessarily reflect the views of HED, USAID, or the United States Government. GB, SC, and DKR acknowledge the financial support of LyondellBasell, LP, the National Science Foundation (CTS # 0626063 to Beaucage), and P&G Corporation. Additional funding to the UCT NanoSciences Innovation Centre was provided by the US Airforce Office of Scientific Research through the project "Nanoparticle Solutions for Printed Electronic Applications", by the University of Cape Town Vice Chancellor's Strategic Fund, and by the South African National Research Foundation (NRF) under focus area grant FA20064160004. The development of the printed silicon materials was supported by the South African Department of Science and Technology through its business unit the Innovation Fund under Technology Advancement Project T50055. ChemMatCARS Sector 15 is principally supported by the National Science Foundation/Department of Energy under grant number NSF/CHE-0822838. Use of the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 42 TC 5 Z9 5 U1 0 U2 17 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 1388-0764 J9 J NANOPART RES JI J. Nanopart. Res. PD NOV PY 2012 VL 14 IS 11 AR 1249 DI 10.1007/s11051-012-1249-y PG 10 WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 030ZG UT WOS:000310608100018 ER PT J AU Mutz, M Eastwood, E Lee, ME Bowen, DE Dadmun, MD AF Mutz, M. Eastwood, Eric Lee, Mark E., Jr. Bowen, Daniel E., III Dadmun, M. D. TI Quantifying the thermodynamic interactions of polyhedral boranes in solution to guide nanocomposite fabrication SO JOURNAL OF NANOPARTICLE RESEARCH LA English DT Article DE Thermodynamics; Light scattering; Boranes; Solubility ID WALLED CARBON NANOTUBES; SOLUBILITY PARAMETERS; ORGANIC-SOLVENTS; DISPERSION; SCATTERING; MOLECULES; LIGHT; C-60 AB The solubility of boron containing nanoparticles in a variety of solvents is quantified using static light scattering in conjunction with refractometry. Four polyhedral boranes were tested in this work, using refractometry to obtain dn/dc, while static light scattering quantifies A(2). A(2) obtained from these measurements was then used to calculate chi, the solute-solvent interaction parameter, and the Hilde-brand solubility parameter, delta, which provides a quantifiable method to identify good solvents. Of the nanoparticles studied, 1,3-di-o-carboranylpropane is thermodynamically stable in toluene, with a chi less than 0.5, a solubility limit of 2.47 mg/mL, and all solutions remaining clear with no visible particle settling. For all of the particles tested, there was good correlation between the physical observations of the solutions, chi, and delta. For instance, lower values of chi correspond to a smaller radius of gyration (R-g). A list of suitable solvents based on delta is also presented. C1 [Mutz, M.; Dadmun, M. D.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Eastwood, Eric; Bowen, Daniel E., III] Honeywell Kansas City Plant, Kansas City, MO USA. [Lee, Mark E., Jr.] Univ Missouri, Columbia, MO 65211 USA. [Dadmun, M. D.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. RP Dadmun, MD (reprint author), Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. EM dad@utk.edu OI Dadmun, Mark/0000-0003-4304-6087 FU Honeywell Federal Manufacturing and Technologies, LLC. FX Funding for this research was provided by Honeywell Federal Manufacturing and Technologies, LLC. NR 38 TC 1 Z9 1 U1 0 U2 10 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 1388-0764 J9 J NANOPART RES JI J. Nanopart. Res. PD NOV PY 2012 VL 14 IS 11 AR 1237 DI 10.1007/s11051-012-1237-2 PG 12 WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA 030ZG UT WOS:000310608100019 ER PT J AU Jun, YC Brener, I AF Jun, Young Chul Brener, Igal TI Electrically tunable infrared metamaterials based on depletion-type semiconductor devices SO JOURNAL OF OPTICS LA English DT Article DE tunable metamaterials; active infrared devices; optoelectronics ID SILICON; FREQUENCY; NANOSTRUCTURES; MODULATOR; INDEX AB We present the theory and experimental demonstration of electrically tunable mid-infrared metamaterials based on depletion-type semiconductor devices. Planar metamaterials consisting of interconnected gold split-ring resonator arrays are fabricated on top of highly doped III-V semiconductors. These arrays work both as an optical metamaterial layer and electrical metal gate simultaneously. The depletion width in the n-doped semiconductor epilayer changes with the electric gate bias, inducing a change of the permittivity of the substrate and leading to frequency tuning of the metamaterial resonance. We first present our device structure and measurement data. Then we provide a detailed theoretical analysis of electrical tuning and we study how semiconductor materials and metamaterial designs affect electrical tunability. We also discuss possible ways to improve tunability even further. This active tuning is generally applicable to a variety of infrared metamaterials and plasmonic structures, which can lead to novel applications in chip-scale infrared optoelectronic devices. C1 [Jun, Young Chul] Sandia Natl Labs, Ctr Integrated Nanotechnol CINT, Albuquerque, NM 87185 USA. RP Jun, YC (reprint author), Sandia Natl Labs, Ctr Integrated Nanotechnol CINT, POB 5800, Albuquerque, NM 87185 USA. EM youngchul.jun@sandia.gov; ibrener@sandia.gov RI Jun, Young Chul/I-2274-2013 OI Jun, Young Chul/0000-0002-7578-8811 FU US Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX We acknowledge Mike Sinclair for his careful reading of the manuscript and insightful comments. We also thank J L Reno and E A Shaner for their support in the experimental part of this work. This work was performed, in part, at the Center for Integrated Nanotechnologies, a US Department of Energy, Office of Basic Energy Sciences user facility. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the US Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 39 TC 15 Z9 16 U1 3 U2 30 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 2040-8978 EI 2040-8986 J9 J OPTICS-UK JI J. Opt. PD NOV PY 2012 VL 14 IS 11 SI SI AR 114013 DI 10.1088/2040-8978/14/11/114013 PG 9 WC Optics SC Optics GA 033YW UT WOS:000310838300014 ER PT J AU Kafesaki, M Shen, NH Tzortzakis, S Soukoulis, CM AF Kafesaki, M. Shen, N. H. Tzortzakis, S. Soukoulis, C. M. TI Optically switchable and tunable terahertz metamaterials through photoconductivity SO JOURNAL OF OPTICS LA English DT Review DE metamaterials; switchable systems; tunable systems; SRRs ID SPLIT-RING RESONATORS; INDEX; REFRACTION AB We present both theoretical and experimental cases for realizing optically switchable and tunable split-ring resonator (SRR) metamaterials operating in the THz regime. This is achieved by suitably placing photoconducting semiconductors in the various SRR designs. Exciting the semiconductor by an optical pump beam, the realization of single- and multi-band switching, blue-shift and red-shift tunability, and broad-band phase modulation are demonstrated. C1 [Kafesaki, M.; Tzortzakis, S.; Soukoulis, C. M.] Fdn Res & Technol Hellas FORTH, Inst Elect Struct & Laser, Iraklion 71110, Crete, Greece. [Kafesaki, M.; Tzortzakis, S.] Univ Crete, Dept Mat Sci & Technol, Iraklion 71003, Crete, Greece. [Shen, N. H.; Soukoulis, C. M.] Iowa State Univ, Ames Lab, USDOE, Ames, IA 50011 USA. [Shen, N. H.; Soukoulis, C. M.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. RP Kafesaki, M (reprint author), Fdn Res & Technol Hellas FORTH, Inst Elect Struct & Laser, POB 1385, Iraklion 71110, Crete, Greece. EM kafesaki@iesl.forth.gr RI Shen, Nianhai/E-5543-2012; Tzortzakis, Stelios/J-5559-2013; Kafesaki, Maria/E-6843-2012; Soukoulis, Costas/A-5295-2008 OI Tzortzakis, Stelios/0000-0001-9242-4182; Kafesaki, Maria/0000-0002-9524-2576; FU EU project PHOME; EU project NIMNIL; EU project ENSEMBLE; COST Action [MP0803]; Department of Energy (Basic Energy Sciences, Division of Materials Sciences and Engineering) [DEAC02-07CH11358] FX We acknowledge financial support by the EU projects PHOME, NIMNIL and ENSEMBLE, and by the COST Action MP0803. Work at Ames Laboratory was supported by the Department of Energy (Basic Energy Sciences, Division of Materials Sciences and Engineering) under Contract No. DEAC02-07CH11358. NR 25 TC 19 Z9 20 U1 6 U2 50 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 2040-8978 J9 J OPTICS-UK JI J. Opt. PD NOV PY 2012 VL 14 IS 11 SI SI AR 114008 DI 10.1088/2040-8978/14/11/114008 PG 8 WC Optics SC Optics GA 033YW UT WOS:000310838300009 ER PT J AU Ma, X Klosterman, L Hu, YY Liu, XP Schmidt-Rohr, K Mallapragada, S Akinc, M AF Ma, Xing Klosterman, Luke Hu, Yan-Yan Liu, Xunpei Schmidt-Rohr, Klaus Mallapragada, Surya Akinc, Mufit TI Aqueous Route Synthesis of Mesoporous ZrO2 by Agarose Templation SO JOURNAL OF THE AMERICAN CERAMIC SOCIETY LA English DT Article ID ZIRCONIA; GELS; OXIDES; POLYSACCHARIDES; COPOLYMER; SILICA AB Mesoporous zirconia with high surface area has been synthesized using self-assembling agarose gel as a template. Agarose gel was formed in the presence of aqueous zirconyl nitrate solutions followed by precipitation of zirconium (hydr)oxide in the gel framework. A porous zirconia structure is obtained by pyrolysis of agarose. Fourier transform infrared spectroscopy is employed to assess the agarose-zirconia precursor interaction. Changes in the C-O absorption bands indicate zirconium association with the OH groups of the agarose. Solid state C-13 NMR studies of the nanocomposite showed a shift in intensity from 70 to 75 ppm indicating conversion of similar to 7% of C-O-H to C-O-Zr. Scanning electron microscopy reveals that both agarose/zirconia nanocomposite and zirconia have similar morphological features as that of pure agarose gel confirming agarose templation. Phase transformation of zirconia from amorphous to tetragonal between 300 degrees C and 500 degrees C, and gradually into monoclinic phase up to 900 degrees C is observed using X-ray powder diffraction. Specific surface area and pore size distribution are determined using nitrogen adsorption, employing BET and BarrettJoynerHalenda methods, respectively. The specific surface area of porous zirconia after heat treatment at 500 degrees C was determined to be 86 m(2)/g, which reduced with increasing temperature to 13 m(2)/g above 900 degrees C. Transmission electron microscopy confirmed the hierarchical structure of porous zirconia. C1 [Ma, Xing; Klosterman, Luke; Hu, Yan-Yan; Liu, Xunpei; Schmidt-Rohr, Klaus; Mallapragada, Surya; Akinc, Mufit] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. [Ma, Xing; Klosterman, Luke; Akinc, Mufit] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. [Hu, Yan-Yan; Schmidt-Rohr, Klaus] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. [Liu, Xunpei; Mallapragada, Surya] Iowa State Univ, Dept Chem & Biol Engn, Ames, IA 50011 USA. RP Akinc, M (reprint author), Iowa State Univ, Ames Lab, Ames, IA 50011 USA. EM makinc@iastate.edu RI Hu, Yan-Yan/A-1795-2015 OI Hu, Yan-Yan/0000-0003-0677-5897 FU U.S. Department of Energy [DE-AC02-07CH11358] FX The work is supported by the U.S. Department of Energy under contract number DE-AC02-07CH11358. NR 41 TC 10 Z9 10 U1 0 U2 50 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0002-7820 EI 1551-2916 J9 J AM CERAM SOC JI J. Am. Ceram. Soc. PD NOV PY 2012 VL 95 IS 11 BP 3455 EP 3462 DI 10.1111/j.1551-2916.2012.05417.x PG 8 WC Materials Science, Ceramics SC Materials Science GA 030WN UT WOS:000310600900019 ER PT J AU Wu, HC Badrinarayanan, P Kessler, MR AF Wu, Hongchao Badrinarayanan, Prashanth Kessler, Michael R. TI Effect of Hydrothermal Synthesis Conditions on the Morphology and Negative Thermal Expansivity of Zirconium Tungstate Nanoparticles SO JOURNAL OF THE AMERICAN CERAMIC SOCIETY LA English DT Article ID PHASE-TRANSITIONS; ZRW2O8 AB Zirconium tungstate (ZrW2O8) is a unique ceramic material that exhibits isotropic negative thermal expansion behavior, which can be produced at relatively low temperatures using hydrothermal synthesis and subsequent heat treatment. In this work, the effect of reaction conditions on morphology and crystallite size of ZrW2O8 nanoparticles is characterized through careful selection of initial reactants, acid types and concentration, reaction time, and temperature. Three types of ZrW2O8 nanoparticles with distinct morphologies and crystallite size scales were chosen to characterize and compare thermal and physical properties. Nano-sized ZrW2O8 particles for two of the morphologies exhibit a negative coefficient of thermal expansion (CTE) that is about 30% larger than the CTE of bulk ZrW2O8 in the alpha-phase (ca. -11.4 vs.-8.8 ppm/degrees C). A dependence of CTE on crystallite size and crystalline structure is demonstrated. It is also found that the morphology of the zirconium tungstate has a significant effect on the pore structure and level of hydration in the nanoparticles. C1 [Wu, Hongchao; Badrinarayanan, Prashanth; Kessler, Michael R.] Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. [Kessler, Michael R.] Iowa State Univ, Dept Mech Engn, Ames, IA USA. [Kessler, Michael R.] US DOE, Ames Lab, Ames, IA 50011 USA. RP Kessler, MR (reprint author), Iowa State Univ, Dept Mat Sci & Engn, Ames, IA 50011 USA. EM mkessler@iastate.edu RI Kessler, Michael/C-3153-2008; Wu, Hongchao/D-4808-2016 OI Kessler, Michael/0000-0001-8436-3447; Wu, Hongchao/0000-0002-0195-8398 FU Honeywell Federal Manufacturing & Technologies LLC; Air Force Office of Scientific Research (AFOSR) FX The authors acknowledge funding from Honeywell Federal Manufacturing & Technologies LLC and the Air Force Office of Scientific Research (AFOSR). We thank Matthew Besser (Ames Laboratory, Ames, IA) for assistance with the isothermal X-ray diffraction measurements, Keenan Deutsch (Chemical Engineering, Iowa State University, Ames, IA) for BET measurements, Tracey Pepper (Genetics, Development & Cell Biology, Iowa State University, Ames, IA) for TEM measurements, and Mohammad Ahmad (Materials Science and Engineering, Iowa State University, Ames, IA) for his suggestion on BET data analysis and XRD pattern refinements. NR 23 TC 8 Z9 8 U1 0 U2 31 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0002-7820 J9 J AM CERAM SOC JI J. Am. Ceram. Soc. PD NOV PY 2012 VL 95 IS 11 BP 3643 EP 3650 DI 10.1111/j.1551-2916.2012.05457.x PG 8 WC Materials Science, Ceramics SC Materials Science GA 030WN UT WOS:000310600900047 ER PT J AU Proffit, DE Ma, Q Buchholz, DB Chang, RPH Bedzyk, MJ Mason, TO AF Proffit, Diana E. Ma, Qing Buchholz, Donald B. Chang, Robert P. H. Bedzyk, Michael J. Mason, Thomas O. TI Structural and Physical Property Studies of Amorphous Zn-In-Sn-O Thin Films SO JOURNAL OF THE AMERICAN CERAMIC SOCIETY LA English DT Article ID TRANSPARENT CONDUCTING OXIDES; X-RAY-SCATTERING; INDIUM-TIN OXIDE; ABSORPTION SPECTROSCOPY; SYNCHROTRON-RADIATION; ELECTRICAL-PROPERTIES; LOCAL-STRUCTURE; IN2O3; BULK; ZITO AB The structures in amorphous (a-) Zn, Sn co-doped In2O3 (ZITO) thin films grown by pulsed laser deposition on glass under varying oxygen pressure or with varying Sn:Zn ratios were determined using X-ray absorption spectroscopy and anomalous X-ray scattering. Typical structures around cations in a-ZITO films are described and compared with crystalline (c-) ZITO films. The results show that the Zn cations are fourfold coordinated with Zn-O bond lengths of 1.98 +/- 0.02 angstrom, which is close to that in bulk ZnO. As a consequence, the second coordination shells around Zn contract. At longer distances away from Zn, the structure is commensurate with the averaged structure. The unit volume around In also contracts slightly compared to bulk In2O3, whereas the Sn-O bond length is similar to the one in bulk SnO2. These unique structural characteristics may account for the films' superior thermal stability over amorphous Sn-doped In2O3, and suggest that Zn and Sn act as network-forming cations. Like in c-ZITO, coordination numbers (N) around Sn, In, and Zn follow the order N-Sn > N-In > N-Zn. Unlike in c-ZITO, where electrical properties change significantly with a slight variation in the Sn:Zn ratio, this variation does not markedly alter the electrical properties, or the local structures, of a-ZITO films. Dramatic changes in the electrical properties occur for films grown under various oxygen pressures, which point to oxygen defects as the source of charge carriers. C1 [Proffit, Diana E.; Buchholz, Donald B.; Chang, Robert P. H.; Bedzyk, Michael J.; Mason, Thomas O.] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. [Ma, Qing] Argonne Natl Lab, Adv Photon Source, NW Synchrotron Res Ctr, DND CAT, Argonne, IL 60439 USA. RP Proffit, DE (reprint author), Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. EM diana.proffit@gmail.com RI Chang, R.P.H/B-7505-2009; Bedzyk, Michael/B-7503-2009; Mason, Thomas/B-7528-2009; Bedzyk, Michael/K-6903-2013 FU NSF MRSEC program at Northwestern University [DMR-1121262]; U.S. Department of Energy, Office of Basic Energy Sciences as part of an Energy Frontier Research Center (DOE) [DE-SC0001059]; NSF Graduate Research Fellowship; E.I. DuPont de Nemours Co.; Dow Chemical Co.; NSF [DMR-9304725]; State of Illinois [IBHE HECA NWU 96]; DOE [DE-AC02-06CH11357] FX This work is supported in part by the NSF MRSEC program at Northwestern University under grant no. DMR-1121262 (DBB, RPHC, MJB, TOM) and in part by the U.S. Department of Energy, Office of Basic Energy Sciences as part of an Energy Frontier Research Center (DOE, grant no. DE-SC0001059, DEP, RPHC, TOM). DEP acknowledges support of an NSF Graduate Research Fellowship. DND-CAT is supported by the E.I. DuPont de Nemours & Co., The Dow Chemical Co., the NSF via grant no. DMR-9304725 (MJB, QM) and the State of Illinois via Grant IBHE HECA NWU 96. The APS is supported by the DOE via Contract no. DE-AC02-06CH11357. The authors acknowledge helpful discussions with C. A. Hoel and K. R. Poeppelmeier. NR 40 TC 13 Z9 13 U1 1 U2 51 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0002-7820 J9 J AM CERAM SOC JI J. Am. Ceram. Soc. PD NOV PY 2012 VL 95 IS 11 BP 3657 EP 3664 DI 10.1111/j.1551-2916.2012.05390.x PG 8 WC Materials Science, Ceramics SC Materials Science GA 030WN UT WOS:000310600900049 ER PT J AU Shinar, J AF Shinar, Joseph TI Optically detected magnetic resonance studies of luminescence-quenching processes in pi-conjugated materials and organic light-emitting devices SO LASER & PHOTONICS REVIEWS LA English DT Article DE OLEDs; photoluminescence quenching processes; electroluminescence quenching processes; triplet exciton-polaron quenching; singlet exciton-polaron quenching; singlet exciton-triplet exciton quenching; bipolarons; trions ID TRIPLET-TRIPLET ANNIHILATION; CONDUCTING POLYMERS; PHOTOEXCITED STATES; TRANSIENT ANALYSIS; POLARON PAIRS; EXCITONS; PHOTOLUMINESCENCE; FILMS; ODMR; ELECTROPHOSPHORESCENCE AB It is widely recognized that nonradiative quenching of excitons by other excitons and polarons become the dominant decay mechanism of these excitons at high excitation densities. These quenching processes cause the roll-off in the efficiency of organic light-emitting devices (OLEDs) and prevent lasing at high injection current densities. This review presents the optically-detected magnetic resonance (ODMR) evidence for these photoluminescence- and electroluminescence-quenching processes. And while it provides such evidence for quenching of singlet excitons by polarons and triplet excitons, it reveals the central role of the strongly spin-dependent annihilation of triplet excitons by polarons, since under normal excitation conditions the steady-state polaron and triplet exciton populations are 100104 times the singlet exciton population. In addition, it also suggests that quenching of singlet excitons by bipolarons, likely stabilized by a counterpolaron or countercharge at specific sites, may also be a significant quenching mechanism that also affects the charge transport properties. C1 [Shinar, Joseph] US DOE, Ames Lab, Ames, IA 50011 USA. [Shinar, Joseph] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. RP Shinar, J (reprint author), US DOE, Ames Lab, Ames, IA 50011 USA. EM jshinar@iastate.edu FU US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division [W-7405-Eng-82, DE-AC 02-07CH11358] FX The author is deeply grateful to the students who conducted the experimental work and the simulations covered in this review, and the colleagues with whom he collaborated on these studies over the past 22 years. Notable former students include Drs. Leland S. Swanson, Paul A. Lane, Adam S. Brown, Andrew V. Smith, Jonathan F. Partee, Willi Graupner, Chang-Hwan Kim, Emil J. W. List, Moon-Ky Lee, and Michael Segal; current students include Ying Chen and Min Cai. Colleagues include Profs. Zeev Valy Vardeny, Eitan Ehrenfreund, Katsumi Yoshino, Thomas J. Barton, Fred Wudl, Donal D. C. Bradley, Richard H. Friend, Lewis J. Rothberg, Esther M. Conwell, Eugene L. Frankevich, Andrei Kadashchuk, Marc A. Baldo, and Zoltan Soos. The work was supported entirely by the US Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division, previously under Contract W-7405-Eng-82 and recently under Contract No. DE-AC 02-07CH11358. NR 81 TC 21 Z9 21 U1 5 U2 52 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1863-8880 EI 1863-8899 J9 LASER PHOTONICS REV JI Laser Photon. Rev. PD NOV PY 2012 VL 6 IS 6 BP 767 EP 786 DI 10.1002/lpor.201100026 PG 20 WC Optics; Physics, Applied; Physics, Condensed Matter SC Optics; Physics GA 030WL UT WOS:000310600700011 ER PT J AU Liu, CC Qi, L Lucks, JB Segall-Shapiro, TH Wang, D Mutalik, VK Arkin, AP AF Liu, Chang C. Qi, Lei Lucks, Julius B. Segall-Shapiro, Thomas H. Wang, Denise Mutalik, Vivek K. Arkin, Adam P. TI An adaptor from translational to transcriptional control enables predictable assembly of complex regulation SO NATURE METHODS LA English DT Article ID SECONDARY STRUCTURE PREDICTION; SINGLE-NUCLEOTIDE RESOLUTION; RNA STRUCTURE-ANALYSIS; GENE-EXPRESSION; SHAPE CHEMISTRY; RIBOSWITCHES; RIBOSOME; RIBOREGULATORS; MECHANISM; FAMILIES AB Bacterial regulators of transcriptional elongation are versatile units for building custom genetic switches, as they control the expression of both coding and noncoding RNAs, act on multigene operons and can be predictably tethered into higher-order regulatory functions (a property called composability). Yet the less versatile bacterial regulators of translational initiation are substantially easier to engineer. To bypass this tradeoff, we have developed an adaptor that converts regulators of translational initiation into regulators of transcriptional elongation in Escherichia coli. We applied this adaptor to the construction of several transcriptional attenuators and activators, including a small molecule-triggered attenuator and a group of five mutually orthogonal riboregulators that we assembled into NOR gates of two, three or four RNA inputs. Continued application of our adaptor should produce large collections of transcriptional regulators whose inherent composability can facilitate the predictable engineering of complex synthetic circuits. C1 [Liu, Chang C.; Qi, Lei; Lucks, Julius B.; Segall-Shapiro, Thomas H.; Wang, Denise; Arkin, Adam P.] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. [Liu, Chang C.; Lucks, Julius B.] Miller Inst Basic Res Sci, Berkeley, CA USA. [Qi, Lei; Arkin, Adam P.] Univ Calif Berkeley, Calif Inst Quantitat Biol Res QB3, Berkeley, CA 94720 USA. [Mutalik, Vivek K.; Arkin, Adam P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Mutalik, Vivek K.; Arkin, Adam P.] Joint BioEnergy Inst JBEI, Emeryville, CA USA. [Arkin, Adam P.] Univ Calif Berkeley, Synthet Biol Inst, Berkeley, CA 94720 USA. RP Arkin, AP (reprint author), Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. EM aparkin@lbl.gov RI Arkin, Adam/A-6751-2008; Lucks, Julius/L-2801-2016; OI Arkin, Adam/0000-0002-4999-2931; Segall-Shapiro, Thomas/0000-0001-9364-6537; Qi, Lei S/0000-0002-3965-3223; Mutalik, Vivek/0000-0001-7934-0400 FU US National Science Foundation, Synthetic Biology Engineering Research Center; Miller Institute for Basic Scientific Research; US Department of Defense through the National Defense Science and Engineering Graduate Fellowship FX We thank C. Yanofsky and M. Samoilov for thoughtful discussions, D. Chen for experimental assistance and S. Meyer for assistance with SHAPE experiments. This work was funded by the US National Science Foundation as part of the Synthetic Biology Engineering Research Center (A. P. A.), the Miller Institute for Basic Scientific Research (C. C. L. and J.B.L.) and the US Department of Defense through the National Defense Science and Engineering Graduate Fellowship (T.H.S.-S.). NR 34 TC 24 Z9 24 U1 0 U2 33 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1548-7091 J9 NAT METHODS JI Nat. Methods PD NOV PY 2012 VL 9 IS 11 BP 1088 EP + DI 10.1038/NMETH.2184 PG 10 WC Biochemical Research Methods SC Biochemistry & Molecular Biology GA 034CW UT WOS:000310848700022 PM 23023598 ER PT J AU Hla, SW AF Hla, Saw Wai TI GRAPHENE Conductivity measurements pick up SO NATURE NANOTECHNOLOGY LA English DT News Item ID NANORIBBONS C1 [Hla, Saw Wai] Ohio Univ, Dept Phys & Astron, Nanoscale & Quantum Phenomena Inst, Athens, OH 45701 USA. [Hla, Saw Wai] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. RP Hla, SW (reprint author), Ohio Univ, Dept Phys & Astron, Nanoscale & Quantum Phenomena Inst, Athens, OH 45701 USA. EM hla@ohio.edu NR 9 TC 1 Z9 1 U1 1 U2 38 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1748-3387 J9 NAT NANOTECHNOL JI Nat. Nanotechnol. PD NOV PY 2012 VL 7 IS 11 BP 693 EP 694 DI 10.1038/nnano.2012.195 PG 2 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA 033JQ UT WOS:000310791900005 PM 23132223 ER PT J AU Oh, J Yuan, HC Branz, HM AF Oh, Jihun Yuan, Hao-Chih Branz, Howard M. TI An 18.2%-efficient black-silicon solar cell achieved through control of carrier recombination in nanostructures SO NATURE NANOTECHNOLOGY LA English DT Article ID PHOTOVOLTAIC APPLICATIONS; SURFACE; ARRAYS; ABSORPTION; NANOWIRES; OXIDATION; VELOCITY AB Silicon nanowire and nanopore arrays promise to reduce manufacturing costs and increase the power conversion efficiency of photovoltaic devices. So far, however, photovoltaic cells based on nanostructured silicon exhibit lower power conversion efficiencies than conventional cells due to the enhanced photocarrier recombination associated with the nanostructures. Here, we identify and separately measure surface recombination and Auger recombination in wafer-based nanostructured silicon solar cells. By identifying the regimes of junction doping concentration in which each mechanism dominates, we were able to design and fabricate an independently confirmed 18.2%-efficient nanostructured 'black-silicon' cell that does not need the antireflection coating layer(s) normally required to reach a comparable performance level. Our results suggest design rules for efficient high-surface-area solar cells with nano-and microstructured semiconductor absorbers. C1 [Oh, Jihun; Yuan, Hao-Chih; Branz, Howard M.] Natl Renewable Energy Lab, Natl Ctr Photovolta, Golden, CO 80401 USA. RP Oh, J (reprint author), Natl Renewable Energy Lab, Natl Ctr Photovolta, 1617 Cole Blvd, Golden, CO 80401 USA. EM jihun.oh@nrel.gov RI Oh, Jihun/B-7085-2013 OI Oh, Jihun/0000-0001-6465-6736 FU DOE American Recovery and Reinvestment Act (ARRA) Photovoltaic Supply Chain and Crosscutting Technologies grant [DE-AC36-08GO28308] FX The authors thank B. To of NREL for assistance with SEM. The authors are grateful to F. Toor and M. R. Page of NREL for many helpful discussions and T. Buonassissi of MIT for important insight into the role of Auger recombination. This work was supported by a DOE American Recovery and Reinvestment Act (ARRA) Photovoltaic Supply Chain and Crosscutting Technologies grant (contract no. DE-AC36-08GO28308). NR 28 TC 296 Z9 303 U1 22 U2 294 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1748-3387 J9 NAT NANOTECHNOL JI Nat. Nanotechnol. PD NOV PY 2012 VL 7 IS 11 BP 743 EP 748 DI 10.1038/NNANO.2012.166 PG 6 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA 033JQ UT WOS:000310791900015 PM 23023643 ER PT J AU Liu, XH Wang, JW Huang, S Fan, FF Huang, X Liu, Y Krylyuk, S Yoo, J Dayeh, SA Davydov, AV Mao, SX Picraux, ST Zhang, SL Li, J Zhu, T Huang, JY AF Liu, Xiao Hua Wang, Jiang Wei Huang, Shan Fan, Feifei Huang, Xu Liu, Yang Krylyuk, Sergiy Yoo, Jinkyoung Dayeh, Shadi A. Davydov, Albert V. Mao, Scott X. Picraux, S. Tom Zhang, Sulin Li, Ju Zhu, Ting Huang, Jian Yu TI In situ atomic-scale imaging of electrochemical lithiation in silicon SO NATURE NANOTECHNOLOGY LA English DT Article ID STRUCTURAL-CHANGES; LITHIUM BATTERIES; ANODES; ELECTRODES; NANOWIRES; FRACTURE; NANOPILLARS; CHALLENGES; ALLOYS AB In lithium-ion batteries, the electrochemical reaction between the electrodes and lithium is a critical process that controls the capacity, cyclability and reliability of the battery. Despite intensive study, the atomistic mechanism of the electrochemical reactions occurring in these solid-state electrodes remains unclear. Here, we show that in situ transmission electron microscopy can be used to study the dynamic lithiation process of single-crystal silicon with atomic resolution. We observe a sharp interface (similar to 1 nm thick) between the crystalline silicon and an amorphous LixSi alloy. The lithiation kinetics are controlled by the migration of the interface, which occurs through a ledge mechanism involving the lateral movement of ledges on the close-packed {111} atomic planes. Such ledge flow processes produce the amorphous LixSi alloy through layer-by-layer peeling of the {111} atomic facets, resulting in the orientation-dependent mobility of the interfaces. C1 [Liu, Xiao Hua; Liu, Yang; Huang, Jian Yu] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA. [Wang, Jiang Wei; Mao, Scott X.] Univ Pittsburgh, Dept Mech Engn & Mat Sci, Pittsburgh, PA 15261 USA. [Huang, Shan; Fan, Feifei; Zhu, Ting] Georgia Inst Technol, George W Woodruff Sch Mech Engn, Atlanta, GA 30332 USA. [Huang, Xu; Zhang, Sulin] Penn State Univ, Dept Engn Sci & Mech, University Pk, PA 16802 USA. [Krylyuk, Sergiy; Davydov, Albert V.] NIST, Mat Measurement Lab, Gaithersburg, MD 20899 USA. [Krylyuk, Sergiy] Univ Maryland, Inst Res Elect & Appl Phys, College Pk, MD 20742 USA. [Yoo, Jinkyoung; Dayeh, Shadi A.; Picraux, S. Tom] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. [Mao, Scott X.] Zhejiang Univ, Ctr Electron Microscopy, Dept Mat Sci & Engn, Hangzhou 310027, Zhejiang, Peoples R China. [Li, Ju] MIT, Dept Nucl Sci & Engn, Cambridge, MA 02139 USA. [Li, Ju] MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA. RP Liu, XH (reprint author), Sandia Natl Labs, Ctr Integrated Nanotechnol, POB 5800, Albuquerque, NM 87185 USA. EM lxhua99@gmail.com; ting.zhu@me.gatech.edu; jyhuang8@yahoo.com RI Li, Ju/A-2993-2008; Zhu, Ting/A-2206-2009; Liu, Xiaohua/A-8752-2011; Wang, Jiangwei/F-8249-2011; Yoo, Jinkyoung/B-5291-2008; Davydov, Albert/F-7773-2010; Zhang, Sulin /E-6457-2010; Liu, Yang/C-9576-2012; Huang, Xu/I-4416-2014; OI Li, Ju/0000-0002-7841-8058; Liu, Xiaohua/0000-0002-7300-7145; Wang, Jiangwei/0000-0003-1191-0782; Yoo, Jinkyoung/0000-0002-9578-6979; Davydov, Albert/0000-0003-4512-2311; Fan, Feifei/0000-0003-0455-4900 FU Laboratory Directed Research and Development (LDRD) project at Sandia National Laboratories (SNL); Nanostructures for Electrical Energy Storage (NEES), an Energy Frontier Research Center (EFRC); US Department of Energy, Office of Science, Office of Basic Energy Sciences [DESC0001160]; US Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; NSF [CMMI-0758554, 1100205, DMR-1008104, DMR-1120901, CMMI-0900692]; AFOSR [FA9550-08-1-0325] FX Portions of this work were supported by a Laboratory Directed Research and Development (LDRD) project at Sandia National Laboratories (SNL) and partly by Nanostructures for Electrical Energy Storage (NEES), an Energy Frontier Research Center (EFRC) funded by the US Department of Energy, Office of Science, Office of Basic Energy Sciences (award no. DESC0001160). The LDRD supported the development and fabrication of platforms. The NEES centre supported the development of TEM techniques. The Sandia-Los Alamos Center for Integrated Nanotechnologies (CINT) supported the TEM capability. Sandia National Laboratories is a multiprogramme laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Company, for the US Department of Energy's National Nuclear Security Administration (contract DE-AC04-94AL85000). T.Z. acknowledges support from the NSF (grants CMMI-0758554 and 1100205). J.L. acknowledges support from the NSF (DMR-1008104 and DMR-1120901) and AFOSR (FA9550-08-1-0325). S.L.Z. acknowledges support from the NSF (grant CMMI-0900692). NR 29 TC 197 Z9 199 U1 30 U2 360 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1748-3387 J9 NAT NANOTECHNOL JI Nat. Nanotechnol. PD NOV PY 2012 VL 7 IS 11 BP 749 EP 756 DI 10.1038/NNANO.2012.170 PG 8 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA 033JQ UT WOS:000310791900016 PM 23042490 ER PT J AU Dromey, B Rykovanov, S Yeung, M Horlein, R Jung, D Gautier, DC Dzelzainis, T Kiefer, D Palaniyppan, S Shah, R Schreiber, J Ruhl, H Fernandez, JC Lewis, CLS Zepf, M Hegelich, BM AF Dromey, B. Rykovanov, S. Yeung, M. Hoerlein, R. Jung, D. Gautier, D. C. Dzelzainis, T. Kiefer, D. Palaniyppan, S. Shah, R. Schreiber, J. Ruhl, H. Fernandez, J. C. Lewis, C. L. S. Zepf, M. Hegelich, B. M. TI Coherent synchrotron emission from electron nanobunches formed in relativistic laser-plasma interactions SO NATURE PHYSICS LA English DT Article ID HARMONIC-GENERATION; SURFACES; PULSE AB Extreme ultraviolet (XUV) and X-ray harmonic spectra produced by intense laser-solid interactions have, so far, been consistent with Doppler upshifted reflection from collective relativistic plasma oscillations-the relativistically oscillating mirror mechanism(1-6). Recent theoretical work, however, has identified a new interaction regime in which dense electron nanobunches are formed at the plasma-vacuum boundary resulting in coherent XUV radiation by coherent synchrotron emission(7,8) (CSE). Our experiments enable the isolation of CSE from competing processes, demonstrating that electron nanobunch formation does indeed occur. We observe spectra with the characteristic spectral signature of CSE-a slow decay of intensity, I, with high-harmonic order, n, as I(n) proportional to n(-1.62) before a rapid efficiency rollover. Particle-in-cell code simulations reveal how dense nanobunches of electrons are periodically formed and accelerated during normal-incidence interactions with ultrathin foils and result in CSE in the transmitted direction. This observation of CSE presents a route to high-energy XUV pulses(7,8) and offers a new window on understanding ultrafast energy coupling during intense laser-solid density interactions. C1 [Dromey, B.; Yeung, M.; Dzelzainis, T.; Lewis, C. L. S.; Zepf, M.] Queens Univ Belfast, Ctr Plasma Phys, Dept Phys & Astron, Belfast BT7 1NN, Antrim, North Ireland. [Rykovanov, S.; Hoerlein, R.; Kiefer, D.; Schreiber, J.; Ruhl, H.] Univ Munich, Dept Phys, D-85748 Garching, Germany. [Hoerlein, R.; Jung, D.; Kiefer, D.; Schreiber, J.; Hegelich, B. M.] Max Planck Inst Quantum Opt, D-85748 Garching, Germany. [Jung, D.; Gautier, D. C.; Palaniyppan, S.; Shah, R.; Fernandez, J. C.; Hegelich, B. M.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Zepf, M.] Helmholtz Inst Jena, D-07743 Jena, Germany. RP Dromey, B (reprint author), Queens Univ Belfast, Ctr Plasma Phys, Dept Phys & Astron, Belfast BT7 1NN, Antrim, North Ireland. EM b.dromey@qub.ac.uk RI Hegelich, Bjorn/J-2689-2013; Fernandez, Juan/H-3268-2011; Zepf, Matt/M-1232-2014 OI Fernandez, Juan/0000-0002-1438-1815; FU EPSRC; Career Acceleration Fellowship FX The authors would like to acknowledge and thank the Trident laser staff for continued support throughout multiple experimental campaigns. B. D. acknowledges support from the EPSRC through grants and a Career Acceleration Fellowship. NR 27 TC 39 Z9 39 U1 2 U2 37 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1745-2473 EI 1745-2481 J9 NAT PHYS JI Nat. Phys. PD NOV PY 2012 VL 8 IS 11 BP 804 EP 808 DI 10.1038/NPHYS2439 PG 5 WC Physics, Multidisciplinary SC Physics GA 033YG UT WOS:000310836700018 ER PT J AU Kugland, NL Ryutov, DD Chang, PY Drake, RP Fiksel, G Froula, DH Glenzer, SH Gregori, G Grosskopf, M Koenig, M Kuramitsu, Y Kuranz, C Levy, MC Liang, E Meinecke, J Miniati, F Morita, T Pelka, A Plechaty, C Presura, R Ravasio, A Remington, BA Reville, B Ross, JS Sakawa, Y Spitkovsky, A Takabe, H Park, HS AF Kugland, N. L. Ryutov, D. D. Chang, P-Y. Drake, R. P. Fiksel, G. Froula, D. H. Glenzer, S. H. Gregori, G. Grosskopf, M. Koenig, M. Kuramitsu, Y. Kuranz, C. Levy, M. C. Liang, E. Meinecke, J. Miniati, F. Morita, T. Pelka, A. Plechaty, C. Presura, R. Ravasio, A. Remington, B. A. Reville, B. Ross, J. S. Sakawa, Y. Spitkovsky, A. Takabe, H. Park, H-S. TI Self-organized electromagnetic field structures in laser-produced counter-streaming plasmas SO NATURE PHYSICS LA English DT Article ID HIGH-POWER LASERS; MAGNETIC-FIELDS; EXPERIMENTAL ASTROPHYSICS; COLLISIONLESS SHOCKS; TURBULENCE; GALAXIES; ELECTRON; FLOWS; BEAMS; JETS AB Self-organization(1,2) occurs in plasmas when energy progressively transfers from smaller to larger scales in an inverse cascade(3). Global structures that emerge from turbulent plasmas can be found in the laboratory(4) and in astrophysical settings; for example, the cosmic magnetic field(5,6,) collisionless shocks in supernova remnants(7) and the internal structures of newly formed stars known as Herbig-Haro objects(8). Here we show that large, stable electromagnetic field structures can also arise within counter-streaming supersonic plasmas in the laboratory. These surprising structures, formed by a yet unexplained mechanism, are predominantly oriented transverse to the primary flow direction, extend for much larger distances than the intrinsic plasma spatial scales and persist for much longer than the plasma kinetic timescales. Our results challenge existing models of counter-streaming plasmas and can be used to better understand large-scale and long-time plasma self-organization. C1 [Kugland, N. L.; Ryutov, D. D.; Glenzer, S. H.; Levy, M. C.; Plechaty, C.; Remington, B. A.; Ross, J. S.; Park, H-S.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Chang, P-Y.; Fiksel, G.; Froula, D. H.] Univ Rochester, Laser Energet Lab, Rochester, NY 14636 USA. [Drake, R. P.; Grosskopf, M.; Kuranz, C.] Univ Michigan, Dept Atmospher Ocean & Space Sci, Ann Arbor, MI 48109 USA. [Gregori, G.; Meinecke, J.; Reville, B.] Univ Oxford, Dept Phys, Oxford OX1 3PU, England. [Koenig, M.; Pelka, A.; Ravasio, A.] Univ Paris 06, Ecole Polytech, LULI, F-91128 Palaiseau, France. [Kuramitsu, Y.; Morita, T.; Sakawa, Y.; Takabe, H.] Osaka Univ, Inst Laser Energet, Suita, Osaka 5650871, Japan. [Levy, M. C.; Liang, E.] Rice Univ, Houston, TX 77251 USA. [Miniati, F.] ETH, Dept Phys, CH-8093 Zurich, Switzerland. [Presura, R.] Univ Nevada, Reno, NV 89557 USA. [Spitkovsky, A.] Princeton Univ, Princeton, NJ 08544 USA. RP Kugland, NL (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM kugland1@llnl.gov RI Chang, Po-Yu/A-9004-2013; Sakawa, Youichi/J-5707-2016; Drake, R Paul/I-9218-2012; Chang, Po-Yu/L-5745-2016 OI Sakawa, Youichi/0000-0003-4165-1048; Drake, R Paul/0000-0002-5450-9844; FU US Department of Energy by the Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; LLNL LDRD [11-ERD-054]; Japan Society for the Promotion of Science; European Research Council under the European Community; ERC [256973, 247039] FX We thank the staff of the OMEGA EP laser facility for their experimental support. This work was performed under the auspices of the US Department of Energy by the Lawrence Livermore National Laboratory, under Contract No. DE-AC52-07NA27344. Further support was provided by LLNL LDRD grant No. 11-ERD-054 and the International Collaboration for High Energy Density Science (ICHEDS), supported by the Core-to-Core Program of the Japan Society for the Promotion of Science. The research leading to these results received funding from the European Research Council under the European Community's Seventh Framework Programme (FP7/2007-2013), ERC grant agreement nos 256973 and 247039. NR 30 TC 51 Z9 52 U1 5 U2 40 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1745-2473 EI 1745-2481 J9 NAT PHYS JI Nat. Phys. PD NOV PY 2012 VL 8 IS 11 BP 809 EP 812 DI 10.1038/NPHYS2434 PG 4 WC Physics, Multidisciplinary SC Physics GA 033YG UT WOS:000310836700019 ER PT J AU Alushin, GM Musinipally, V Matson, D Tooley, J Stukenberg, PT Nogales, E AF Alushin, Gregory M. Musinipally, Vivek Matson, Daniel Tooley, John Stukenberg, P. Todd Nogales, Eva TI Multimodal microtubule binding by the Ndc80 kinetochore complex SO NATURE STRUCTURAL & MOLECULAR BIOLOGY LA English DT Article ID ELECTRON-MICROSCOPY; SKA COMPLEX; CHROMOSOME CONGRESSION; OUTER KINETOCHORE; YEAST KINETOCHORE; NEW-GENERATION; ATTACHMENT; RESOLUTION; COMPONENT; HEC1 AB The Ndc80 complex is a key site of kinetochore-microtubule attachment during cell division. The human complex engages microtubules with a globular 'head' formed by tandem calponin-homology domains and an 80-amino-acid unstructured 'tail' that contains sites of phosphoregulation by the Aurora B kinase. Using biochemical, cell biological and electron microscopy analyses, we dissected the roles of the tail in binding of microtubules and mediation of cooperative interactions between Ndc80 complexes. Two segments of the tail that contain Aurora B phosphorylation sites become ordered at interfaces; one with tubulin and the second with an adjacent Ndc80 head on the microtubule surface, forming interactions that are disrupted by phosphorylation. We propose a model in which Ndc80's interaction with either growing or shrinking microtubule ends can be tuned by the phosphorylation state of its tail. C1 [Nogales, Eva] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. [Alushin, Gregory M.] Univ Calif Berkeley, Biophys Grad Grp, Berkeley, CA 94720 USA. [Nogales, Eva] Univ Calif Berkeley, Dept Mol & Cell Biol, Howard Hughes Med Inst, Berkeley, CA 94720 USA. [Matson, Daniel; Tooley, John; Stukenberg, P. Todd] Univ Virginia, Sch Med, Dept Biochem & Mol Genet, Charlottesville, VA 22908 USA. RP Nogales, E (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. EM enogales@lbl.gov OI Stukenberg, Todd/0000-0002-6788-2111 FU US National Institutes of Health [GM051487, GM081576]; Howard Hughes Medical Institute FX We acknowledge G. Lander for assistance with image processing. GST tail expression constructs were generated by members of the QB3 Macrolab at University of California Berkeley. We thank T. Houweling, P. Grob and G. Kemalyan for computer and electron microscopy support. G.M.A. is partially supported by a US National Institutes of Health training grant. This work was funded by grants from the US National Institutes of Health (GM051487 to E.N. and GM081576 to P.T.S.). E.N. is also funded by the Howard Hughes Medical Institute. NR 58 TC 33 Z9 34 U1 0 U2 11 PU NATURE PUBLISHING GROUP PI NEW YORK PA 75 VARICK ST, 9TH FLR, NEW YORK, NY 10013-1917 USA SN 1545-9993 J9 NAT STRUCT MOL BIOL JI Nat. Struct. Mol. Biol. PD NOV PY 2012 VL 19 IS 11 BP 1161 EP + DI 10.1038/nsmb.2411 PG 9 WC Biochemistry & Molecular Biology; Biophysics; Cell Biology SC Biochemistry & Molecular Biology; Biophysics; Cell Biology GA 033IT UT WOS:000310788800016 PM 23085714 ER PT J AU Reich, CW AF Reich, C. W. TI Nuclear Data Sheets for A=156 SO NUCLEAR DATA SHEETS LA English DT Article ID HIGH-SPIN STATES; RARE-EARTH NUCLEI; ODD-ODD NUCLEI; GAMMA-RAY SPECTROSCOPY; REDUCED TRANSITION-PROBABILITIES; NEUTRON-DEFICIENT ISOTOPES; INTERACTING BOSON MODEL; COLLECTIVE VIBRATIONAL STATES; INELASTIC ELECTRON-SCATTERING; INTERNAL-CONVERSION LINES AB All the known nuclear-structure information on the A=156 nuclides from Nd-156 through Ta-156 has been reviewed. These data are summarized and presented, together with adopted level schemes and properties based on an evaluation of them. C1 Brookhaven Natl Lab, Natl Nucl Data Ctr, Upton, NY 11973 USA. RP Reich, CW (reprint author), Brookhaven Natl Lab, Natl Nucl Data Ctr, Upton, NY 11973 USA. FU U. S. Department of Energy; National Nuclear Data Center at the Brookhaven National Laboratory FX Work supported by the U. S. Department of Energy under a contract with the National Nuclear Data Center at the Brookhaven National Laboratory. NR 504 TC 14 Z9 14 U1 1 U2 13 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0090-3752 J9 NUCL DATA SHEETS JI Nucl. Data Sheets PD NOV PY 2012 VL 113 IS 11 BP 2537 EP 2840 PG 304 WC Physics, Nuclear SC Physics GA 032ZW UT WOS:000310763000001 ER PT J AU Ferrieri, AP Appel, H Ferrieri, RA Schultz, JC AF Ferrieri, Abigail P. Appel, Heidi Ferrieri, Richard A. Schultz, Jack C. TI Novel application of 2-[F-18]fluoro-2-deoxy-D-glucose to study plant defenses SO NUCLEAR MEDICINE AND BIOLOGY LA English DT Article DE 2-[F-18]fluoro-2-deoxy-D-glucose; Arabidopsis thaliana; Methyl jasmonate; Metabolic partitioning; Short-lived radiotracers; Competing sinks ID METHYL JASMONATE; ARABIDOPSIS-THALIANA; RAPID CHANGES; NICOTIANA-ATTENUATA; CARBON TRANSPORT; GENE-EXPRESSION; LEAVES; INDUCTION; TRANSLOCATION; BIOSYNTHESIS AB Introduction: Since its first use in humans in 1976, 2-[F-18]fluoro-2-deoxy-D-glucose ((18)FDG) continues to serve as a tracer to measure tissue glucose metabolism in medical imaging. Here we demonstrate a novel use for this tracer to study glycoside biosynthesis in plants as a measure of plant response to defense induction. Methods: Coupling autoradiography with radio high-performance liquid chromatography analysis of tissue extracts, we examined the combined effects of leaf wounding and treatment using the potent plant defense hormone, methyl jasmonate (MeJA), to measure tracer distribution and tracer use in secondary defense chemistry in Arabidopsis thaliana. We hypothesized that competing sinks like roots and reproductive tissues, as well as vascular architecture, would impact the induction of phenolic defenses of the plant that make use of glucose in glycoside formation by altering distribution and metabolic utilization of (18)FDG. Results: Our studies showed that leaf orthostichy defined the major route of (18)FDG transport in both vegetative and reproductive plants when a single petiole was cut as the entry point for tracer introduction. However, when nonorthostichous leaves were damaged and treated with MeJA, (18)FDG was transported in its intact form to these leaves 3 h later, where it was incorporated into phenolic glycosides. Conclusions: Our work demonstrates a new use for (18)FDG in plant science with insights into carbohydrate allocation that contradict conclusions of previous studies showing transport of resources away from damaged sites. (C) 2012 Elsevier Inc. All rights reserved. C1 [Ferrieri, Abigail P.; Appel, Heidi; Schultz, Jack C.] Univ Missouri, Bond Life Sci Ctr, Div Plant Sci, Columbia, MO 65211 USA. [Ferrieri, Richard A.] Brookhaven Natl Lab, Dept Med, Upton, NY 11973 USA. RP Ferrieri, AP (reprint author), Univ Missouri, Bond Life Sci Ctr, Div Plant Sci, Columbia, MO 65211 USA. EM apfvfb@mail.missouri.edu OI Schultz, Jack/0000-0001-9870-3537 FU US Department of Energy, Office of Biological and Environmental Research [DE-AC02-98CH10886]; University of Missouri, Chemistry Department [DOE DE-SC0002040]; National Science Foundation [IOS-0805272]; MU Life Sciences Fellowship Program FX We thank M. Kasel for methods related to 18FDG desalination, as well as other members of the Schultz-Appel lab for insightful comments that improved this manuscript. This research was supported by the US Department of Energy, Office of Biological and Environmental Research under contract DE-AC02-98CH10886 to R.A.F.; DOE DE-SC0002040 Research Projects for Interrogations of Biological Systems: Training for the Development of Novel Radiotracer (University of Missouri, Chemistry Department), National Science Foundation grant IOS-0805272 to J.S. and HA.; and the MU Life Sciences Fellowship Program, which supported A. Ferrieri. NR 59 TC 17 Z9 18 U1 0 U2 15 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 0969-8051 J9 NUCL MED BIOL JI Nucl. Med. Biol. PD NOV PY 2012 VL 39 IS 8 BP 1152 EP 1160 DI 10.1016/j.nucmedbio.2012.06.005 PG 9 WC Radiology, Nuclear Medicine & Medical Imaging SC Radiology, Nuclear Medicine & Medical Imaging GA 031VZ UT WOS:000310672000008 PM 22795788 ER PT J AU Liao, ZM Roussell, R Adams, JJ Runkel, M Frenk, WT Luken, J Carr, CW AF Liao, Zhi M. Roussell, R. Adams, J. J. Runkel, M. Frenk, W. T. Luken, J. Carr, C. W. TI Defect population variability in deuterated potassium di-hydrogen phosphate crystals SO OPTICAL MATERIALS EXPRESS LA English DT Article ID LASER-INDUCED DAMAGE; GROWN KDP CRYSTALS; BULK DAMAGE; KH2PO4 AB Bulk laser damage variability in deuterated potassium dihydrogen phosphate (DKDP) crystals is well known and makes online conditioning of multiple-beam laser systems difficult to optimize. By using an empirical model, called Absorption Distribution Model (ADM), we were able to map the damage variability of the crystals (boule to boule as well as within same boule) in terms of defect population variations. The defect population variation was found to coalesce into two distinct groupings that can be identified by the defect population in the late growth region of the boule. This result allows us to optimize the conditioning protocol for an arbitrary number of beams with crystals of differing damage quality. (C) 2012 Optical Society of America C1 [Liao, Zhi M.; Adams, J. J.; Runkel, M.; Carr, C. W.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Roussell, R.] Southern Univ, Baton Rouge, LA 70813 USA. [Frenk, W. T.; Luken, J.] Gooch & Husego Ohio LLC, Highland Hts, OH 44143 USA. [Roussell, R.] A&M Coll, Baton Rouge, LA 70813 USA. RP Liao, ZM (reprint author), Lawrence Livermore Natl Lab, 7000 E Ave, Livermore, CA 94550 USA. EM zman@llnl.gov RI Carr, Chris/F-7163-2013; Liao, Zhi/G-3729-2013 FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; LLNL office of LDRD [LLNL-JRNL-576732] FX The authors thank Cindy Cassady for help in editing this manuscript. This work is performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344 and funded through LLNL office of LDRD (LLNL-JRNL-576732). NR 21 TC 4 Z9 5 U1 0 U2 22 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 2159-3930 J9 OPT MATER EXPRESS JI Opt. Mater. Express PD NOV 1 PY 2012 VL 2 IS 11 BP 1612 EP 1623 PG 12 WC Materials Science, Multidisciplinary; Optics SC Materials Science; Optics GA 031NB UT WOS:000310647500017 ER PT J AU Wright, JB Cicotte, KN Subramania, G Dirk, SM Brener, I AF Wright, Jeremy B. Cicotte, Kirsten N. Subramania, Ganapathi Dirk, Shawn M. Brener, Igal TI Chemoselective gas sensors based on plasmonic nanohole arrays SO OPTICAL MATERIALS EXPRESS LA English DT Article ID EXTRAORDINARY OPTICAL-TRANSMISSION; SUBWAVELENGTH HOLE ARRAYS; ELECTROCHEMICAL DETECTION; ELECTRODE ARRAYS; ANTIBODIES; RESONANCE; LIGHT AB We have demonstrated a binary chemoselective gas sensor using a combination of plasmonic nanohole arrays and a voltage-directed assembly of diazonium chemistry. The employment of a voltage-directed functionalization allows for the realization of a multiplexed sensor. The device was read optically and was fabricated using a combination of electron-beam and conventional lithography; it contains several regions each electrically isolated from each other. We used calibrated gas dosage delivery to confirm the selectivity of the sensor and observed reversible spectral shifts of several nm upon gas exposure. The resulting spectral shift indicates the potential for use in chemical arrayed detection for low concentration gas sensing (C) 2012 Optical Society of America C1 [Wright, Jeremy B.; Cicotte, Kirsten N.; Dirk, Shawn M.] Sandia Natl Labs, Organ Mat Dept, Albuquerque, NM 87185 USA. [Subramania, Ganapathi; Brener, Igal] Sandia Natl Labs, Ctr Integrated Nanotechnol, Albuquerque, NM 87185 USA. RP Wright, JB (reprint author), Sandia Natl Labs, Organ Mat Dept, 1515 Eubank SE, Albuquerque, NM 87185 USA. EM ibrener@sandia.gov RI Wright, Jeremy/G-7149-2011 OI Wright, Jeremy/0000-0001-6861-930X FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was performed, in part, at the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences user facility. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 19 TC 10 Z9 10 U1 2 U2 26 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 2159-3930 J9 OPT MATER EXPRESS JI Opt. Mater. Express PD NOV 1 PY 2012 VL 2 IS 11 BP 1655 EP 1662 PG 8 WC Materials Science, Multidisciplinary; Optics SC Materials Science; Optics GA 031NB UT WOS:000310647500021 ER PT J AU Spagnolo, V Patimisco, P Borri, S Scamarcio, G Bernacki, BE Kriesel, J AF Spagnolo, Vincenzo Patimisco, Pietro Borri, Simone Scamarcio, Gaetano Bernacki, Bruce E. Kriesel, Jason TI Part-per-trillion level SF6 detection using a quartz enhanced photoacoustic spectroscopy-based sensor with single-mode fiber-coupled quantum cascade laser excitation SO OPTICS LETTERS LA English DT Article AB A sensitive spectroscopic sensor based on a hollow-core fiber-coupled quantum cascade laser (QCL) emitting at 10.54 mu m and quartz enhanced photoacoustic spectroscopy (QEPAS) technique is reported. The design and realization of mid-IR fiber and coupler optics has ensured single-mode QCL beam delivery to the QEPAS sensor. The collimation optics was designed to produce a laser beam of significantly reduced beam size and waist so as to prevent illumination of the quartz tuning fork and microresonator tubes. SF6 was selected as the target gas. A minimum detection sensitivity of 50 parts per trillion in 1 s was achieved with a QCL power of 18 mW, corresponding to a normalized noise-equivalent absorption of 2.7 x 10(-10) W . cm(-1)/Hz(1/2). (C) 2012 Optical Society of America C1 [Spagnolo, Vincenzo; Patimisco, Pietro; Borri, Simone; Scamarcio, Gaetano] Univ Bari, Dipartimento Interateneo Fis, I-70100 Bari, Italy. [Spagnolo, Vincenzo; Patimisco, Pietro; Borri, Simone; Scamarcio, Gaetano] Politecn Bari, CNR IFN UOS BARI, I-70100 Bari, Italy. [Bernacki, Bruce E.] Pacific NW Natl Lab, Richland, WA 99354 USA. [Kriesel, Jason] Optoknowledge Syst Inc, Torrance, CA 90502 USA. RP Spagnolo, V (reprint author), Univ Bari, Dipartimento Interateneo Fis, Via Amendola 173, I-70100 Bari, Italy. EM spagnolo@fisica.uniba.it RI Scamarcio, Gaetano/I-7674-2014; OI Scamarcio, Gaetano/0000-0003-0808-4336; Borri, Simone/0000-0001-8471-2803; Spagnolo, Vincenzo/0000-0002-4867-8166 FU [PON01_02238]; [PON02_00675] FX The authors acknowledge financial support from the Italian research projects: PON01_02238 and PON02_00675. NR 15 TC 52 Z9 54 U1 4 U2 54 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 0146-9592 J9 OPT LETT JI Opt. Lett. PD NOV 1 PY 2012 VL 37 IS 21 BP 4461 EP 4463 PG 3 WC Optics SC Optics GA 030NP UT WOS:000310577700036 PM 23114329 ER PT J AU Wengraitis, S Reed, NG AF Wengraitis, Stephen Reed, Nicholas G. TI Ultraviolet Spectral Reflectance of Ceiling Tiles, and Implications for the Safe Use of Upper-Room Ultraviolet Germicidal Irradiation SO PHOTOCHEMISTRY AND PHOTOBIOLOGY LA English DT Article ID AIR DISINFECTION; HISTORY AB Ultraviolet germicidal irradiation can be used to prevent airborne transmission of infectious diseases. A common application is to irradiate upper-room areas, by passing air from the lower room into the irradiated zone. Well-designed systems do not expose people directly; however, some UV radiation may be reflected off ceiling tiles and wall paints into the lower room. Lower room exposure should be limited to the American Conference of Governmental Industrial Hygienists threshold limit value of 6 mJ center dot cm(-2) of 254 nm radiation per day. To limit the lower room exposure, the reflectance of upper-room surfaces must not be high. The reflective properties of wall paints have been studied, but less is known about the UV reflectance of ceiling tiles. Using a double monochromator spectroradiometer and an integrating sphere reflectance attachment, the UV spectral reflectance of 37 ceiling tiles was measured from 200 to 400 nm. The reflectances varied from 0.020 to 0.822 in this range, and from 0.035 to 0.459 at 254 nm, the main wavelength emitted by upper room low-pressure mercury germicidal lamps. These data were then used to estimate an 8 h exposure based on several simplified workplace scenarios. The implications for workplace safety are then discussed. C1 [Wengraitis, Stephen] USA, Publ Hlth Command, MCHB IP OLO, Aberdeen Proving Ground, MD USA. [Reed, Nicholas G.] ORAU ORISE Maryland, Belcamp, MD USA. RP Wengraitis, S (reprint author), USA, Publ Hlth Command, MCHB IP OLO, Aberdeen Proving Ground, MD USA. EM steve.wengraitis@mail.us.army.mil FU U.S. Department of Energy; US-APHC FX This project was supported in part by an appointment to the Internship/Research Participation Program for the US Army Public Health Command (USAPHC) administered by the Oak Ridge Institute for Science and Education through an agreement between the U.S. Department of Energy and the US-APHC. The views expressed in this article are the views of the authors and do not reflect the official policy or position of the Department of the Army, the Department of Defense, or the U.S. government. Use of trademarked name does not imply endorsement by the U.S. Army, but is intended only to assist in identification of a specific product. NR 32 TC 3 Z9 3 U1 1 U2 7 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0031-8655 J9 PHOTOCHEM PHOTOBIOL JI Photochem. Photobiol. PD NOV-DEC PY 2012 VL 88 IS 6 BP 1480 EP 1488 DI 10.1111/j.1751-1097.2012.01193.x PG 9 WC Biochemistry & Molecular Biology; Biophysics SC Biochemistry & Molecular Biology; Biophysics GA 030IB UT WOS:000310563300020 PM 22731691 ER PT J AU Matlashov, AN Burmistrov, E Magnelind, PE Schultz, L Urbaitis, AV Volegov, PL Yoder, J Espy, MA AF Matlashov, A. N. Burmistrov, E. Magnelind, P. E. Schultz, L. Urbaitis, A. V. Volegov, P. L. Yoder, J. Espy, M. A. TI SQUID-based systems for co-registration of ultra-low field nuclear magnetic resonance images and magnetoencephalography SO PHYSICA C-SUPERCONDUCTIVITY AND ITS APPLICATIONS LA English DT Article DE MRI; ULF; Microtesla; Low-field MRI; MEG; SQUID ID HUMAN BRAIN; MRI; NMR; INSTRUMENTATION; NOISE AB The ability to perform magnetic resonance imaging (MRI) in ultra-low magnetic fields (ULF) of similar to 100 mu T, using superconducting quantum interference device (SQUID) detection, has enabled a new class of magnetoencephalography (MEG) instrumentation capable of recording both anatomical (via the ULF MRI) and functional (biomagnetic) information about the brain. The combined ULF MRI/MEG instrument allows both structural and functional information to be co-registered to a single coordinate system and acquired in a single device. In this paper we discuss the considerations and challenges required to develop a combined ULF MRI/MEG device, including pulse sequence development, magnetic field generation, SQUID operation in an environment of pulsed pre-polarization, and optimization of pick-up coil geometries for MRI in different noise environments. We also discuss the design of a "hybrid" ULF MRI/MEG system under development in our laboratory that uses SQUID pick-up coils separately optimized for MEG and ULF MRI. Published by Elsevier B.V. C1 [Matlashov, A. N.; Burmistrov, E.; Magnelind, P. E.; Schultz, L.; Urbaitis, A. V.; Volegov, P. L.; Yoder, J.; Espy, M. A.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Matlashov, AN (reprint author), Los Alamos Natl Lab, POB 1663,MS-D454, Los Alamos, NM 87545 USA. EM matlach@lanl.gov OI Urbaitis, Algis/0000-0002-8626-5987 FU LANL's LDRD office [20100097DR] FX The authors thank John Gomez, Shaun Newman, Henrik Sandin, and Robert Sedillo for their significant efforts in turning our design into a real system. We would also like to thank Joseph Schillig for his modeling contribution to the design and optimization of the field generation hardware presented here. We gratefully acknowledge the support from LANL's LDRD office through the Grant 20100097DR. NR 23 TC 12 Z9 12 U1 1 U2 22 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0921-4534 J9 PHYSICA C JI Physica C PD NOV PY 2012 VL 482 BP 19 EP 26 DI 10.1016/j.physc.2012.04.028 PG 8 WC Physics, Applied SC Physics GA 033HE UT WOS:000310784100003 ER PT J AU Chu, CW AF Chu, C. W. TI A possible approach from BCS through HTS to RTS with three examples SO PHYSICA C-SUPERCONDUCTIVITY AND ITS APPLICATIONS LA English DT Article DE High temperature superconductivity; Very high temperature superconductivity; Room temperature superconductivity; Novel superconducting mechanisms; New superconducting compounds ID CU-O SYSTEM; HIGH-TEMPERATURE SUPERCONDUCTIVITY; BAPB1-XBIXO3 SYSTEM; EXCITON MECHANISM; COMPOUND SYSTEM; DEGREES K; PRESSURE; TRANSITION; LA; SURFACE AB This paper is based on my talk delivered at the superconductivity centennial conference in The Hague, the Netherlands, on September 23, 2011, to explore the possibility of room temperature superconductivity according to what we have learned from the past, especially in the last 25 years since the discovery of high temperature superconductivity. While the field of superconductivity is broad, I have chosen to focus on the advancement of T-c, which has been a major driving force for sustaining research on superconductivity for the last 100 years, ever since its discovery by Heike Kamerlingh Onnes in Leiden. A holistic multidisciplinary enlightened empirical approach is proposed with some specific steps following a brief summary of the past history in the search for superconductors with higher T-c. Before concluding, three specific examples of our effort toward superconductors of higher T-c are given to demonstrate that the future in raising T-c is vast and bright. (C) 2012 Elsevier B.V. All rights reserved. C1 [Chu, C. W.] Univ Houston, Dept Phys, Houston, TX 77204 USA. [Chu, C. W.] Univ Houston, Texas Ctr Superconduct, Houston, TX 77204 USA. [Chu, C. W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Chu, CW (reprint author), Univ Houston, Dept Phys, Houston, TX 77204 USA. EM cwchu@uh.edu FU AFOSR; DoE; AFRL (CONTACT); T.L. L. Temple Foundation; John J. and Rebecca Moores Foundation; State of Texas FX I would like to thank the Chairmen of the Conference, Professors Horst Rogalla and Peter Kes, for inviting me to participate in this spectacular scientific feast in the Netherlands where the epoch discovery was made 100 years ago by Heike Kamerlingh Onnessurely a special honor and privilege for me, as a practitioner in the field for decades. I would also like to express my gratitude to colleagues at TCSUH, B. Lv, Y. Y. Xue, L. Z. Deng, F. Y. Wei, M. Gooch, J. Meen, and B. Lorenz, for technical assistance and discussion. The work in Houston is supported in part by AFOSR, DoE, AFRL (CONTACT), the T.L. L. Temple Foundation, the John J. and Rebecca Moores Foundation, and the State of Texas. NR 84 TC 7 Z9 7 U1 2 U2 38 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0921-4534 J9 PHYSICA C JI Physica C PD NOV PY 2012 VL 482 BP 33 EP 44 DI 10.1016/j.physc.2012.04.033 PG 12 WC Physics, Applied SC Physics GA 033HE UT WOS:000310784100005 ER PT J AU Yu, ZH Li, CY Liu, HZ AF Yu, Z. H. Li, C. Y. Liu, H. Z. TI In situ high-pressure synchrotron X-ray diffraction study of the structural stability in the intermetallic compound Mn2Sb SO PHYSICA STATUS SOLIDI B-BASIC SOLID STATE PHYSICS LA English DT Article DE crystal structure and symmetry; intermetallic compounds; magnetically ordered materials; Mn2Sb; phase transitions; X-ray diffraction ID MAGNETIC TRANSITION-TEMPERATURE; CHROMIUM-MODIFIED MN2SB; CR-MODIFIED MN2SB; METAMAGNETIC-TRANSITION; NEUTRON-DIFFRACTION; LATTICE-PARAMETERS; PHASE-TRANSITION; MN2-XCOXSB; CRYSTALS; GAUGE AB Cu2Sb-type (Strukturbericht designation: C38) intermetallic compound Mn2Sb was studied up to 25.7?GPa at room temperature using the in situ synchrotron powder X-ray diffraction (XRD) technique. Our results from the XRD analysis showed that the (C38)-type Mn2Sb undergoes a pressure-induced structural phase transition near 22.4?GPa. In the low-pressure (LP) phase of Mn2Sb, an anisotropic compressibility was observed with greater compressibility along the a-axis than the c-axis. And the mechanism for the anisotropy of compressibility was discussed in terms of the stacking of crystallography. Fitted to a third-order BirchMurnaghan equation of state (BM-EOS), the pressurevolume data of Mn2Sb yielded the stable lattice volume V0?=?109.45(3)?angstrom 3, bulk modulus B0?=?50.1(5)?GPa, and its derivative $B'_{{\rm 0}} $?=?7.0(2) for the LP phase. We propose that the distortion of Mn(I)Sb4 tetrahedra may give rise to the structural instability of Mn2Sb under high pressure (HP). C1 [Yu, Z. H.; Li, C. Y.] Harbin Inst Technol, Dept Phys, Harbin 150080, Peoples R China. [Yu, Z. H.] Argonne Natl Lab, XSD, Adv Photon Source, Argonne, IL 60439 USA. [Li, C. Y.] Brookhaven Natl Lab, Photon Sci Directorate, Upton, NY 11973 USA. [Liu, H. Z.] Harbin Inst Technol, Nat Sci Res Ctr, Harbin 150080, Peoples R China. RP Yu, ZH (reprint author), Harbin Inst Technol, Dept Phys, Harbin 150080, Peoples R China. EM zhenhaiuy@gmail.com RI Liu, Haozhe/E-6169-2011 FU COMPRES (the Consortium for Materials Properties Research in Earth Sciences); China Scholarship Council FX Thanks to Dr. Zhiqiang Chen for the experimental help. We acknowledge the National Synchrotron Light Source (NSLS) of Brookhaven National Laboratory (BNL) for the provision of synchrotron radiation facilities beam line X17C. We are thankful for support from COMPRES (the Consortium for Materials Properties Research in Earth Sciences). This work was partly supported by China Scholarship Council. We are grateful to the editor and anonymous referees for their thorough reading of the paper and suggestion for improvement. NR 31 TC 0 Z9 0 U1 1 U2 21 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0370-1972 EI 1521-3951 J9 PHYS STATUS SOLIDI B JI Phys. Status Solidi B-Basic Solid State Phys. PD NOV PY 2012 VL 249 IS 11 BP 2239 EP 2243 DI 10.1002/pssb.201248182 PG 5 WC Physics, Condensed Matter SC Physics GA 033IW UT WOS:000310789200026 ER PT J AU Tiburzi, BC AF Tiburzi, B. C. TI Isotensor hadronic parity violation SO PHYSICAL REVIEW D LA English DT Article ID NONLEPTONIC DECAYS; WEAK DECAYS; DELTA-S=1; QCD AB Weak interactions between quarks give rise to hadronic parity violation which can be observed in nuclear and few-nucleon systems. We study the QCD renormalization of the isotensor component of parity violation at next-to-leading order accuracy. The renormalization group is employed to evolve the interaction down to hadronic scales. As the results are renormalization-scheme dependent, we compare various schemes, including 't Hooft-Veltman dimensional regularization and several regularization-independent momentum subtraction schemes. C1 [Tiburzi, B. C.] CUNY City Coll, Dept Phys, New York, NY 10031 USA. [Tiburzi, B. C.] CUNY Grad Sch & Univ Ctr, New York, NY 10016 USA. [Tiburzi, B. C.] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. RP Tiburzi, BC (reprint author), CUNY City Coll, Dept Phys, New York, NY 10031 USA. EM btiburzi@ccny.cuny.edu OI Tiburzi, Brian/0000-0001-8696-2902 FU CCNY-RBRC; U.S. National Science Foundation [PHY-1205778] FX Work supported in part by a joint CCNY-RBRC fellowship and the U.S. National Science Foundation, under Grant No. PHY-1205778. NR 27 TC 1 Z9 1 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 J9 PHYS REV D JI Phys. Rev. D PD NOV 1 PY 2012 VL 86 IS 9 AR 097501 DI 10.1103/PhysRevD.86.097501 PG 5 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 029MS UT WOS:000310500500017 ER PT J AU Chiu, TY Christiansen, K Moreno, I Lao, JM Loque, D Orellana, A Heazlewood, JL Clark, G Roux, SJ AF Chiu, Tsan-Yu Christiansen, Katy Moreno, Ignacio Lao, Jeemeng Loque, Dominique Orellana, Ariel Heazlewood, Joshua L. Clark, Greg Roux, Stanley J. TI AtAPY1 and AtAPY2 Function as Golgi-Localized Nucleoside Diphosphatases in Arabidopsis thaliana SO PLANT AND CELL PHYSIOLOGY LA English DT Article DE Arabidopsis; Functional complementation; Golgi NTPDase; Glycosylation ID YEAST SECRETORY PATHWAY; CELL-WALL BIOSYNTHESIS; EXTRACELLULAR ATP; SACCHAROMYCES-CEREVISIAE; PEA STEMS; POLYSACCHARIDE BIOSYNTHESIS; GUANOSINE DIPHOSPHATASE; MEDICAGO-TRUNCATULA; GDP-MANNOSE; RAT-LIVER AB Nucleoside triphosphate diphosphohydrolases (NTPDases; apyrases) (EC 3.6.1.5) hydrolyze di- and triphosphate nucleotides, but not monophosphate nucleotides. They are categorized as E-type ATPases, have a broad divalent cation (Mg2+, Ca2+) requirement for activation and are insensitive to inhibitors of F-type, P-type and V-type ATPases. Among the seven NTPDases identified in Arabidopsis, only APYRASE 1 (AtAPY1) and APYRASE 2 (AtAPY2) have been previously characterized. In this work, either AtAPY1 or AtAPY2 tagged with C-terminal green fluorescent protein (GFP) driven by their respective native promoter can rescue the apy1 apy2 double knockout (apy1 apy2 dKO) successfully, and confocal microscopy reveals that these two Arabidopsis apyrases reside in the Golgi apparatus. In Saccharomyces cerevisiae, both AtAPY1 and AtAPY2 can complement the Golgi-localized GDA1 mutant, rescuing its aberrant protein glycosylation phenotype. In Arabidopsis, microsomes of the wild type show higher substrate preferences toward UDP compared with other NDP substrates. Loss-of-function Arabidopsis AtAPY1 mutants exhibit reduced microsomal UDPase activity, and this activity is even more significantly reduced in the loss-of-function AtAPY2 mutant and in the AtAPY1/AtAPY2 RNA interference (RNAi) technology repressor lines. Microsomes from wild-type plants also have detectable GDPase activity, which is significantly reduced in apy2 but not apy1 mutants. The GFP-tagged AtAPY1 or AtAPY2 constructs in the apy1 apy2 dKO plants can restore microsomal UDP/GDPase activity, confirming that they both also have functional competency. The cell walls of apy1, apy2 and the RNAi-silenced lines all have an increased composition of galactose, but the transport efficiency of UDP-galactose across microsomal membranes was not altered. Taken together, these results reveal that AtAPY1 and AtAPY2 are Golgi-localized nucleotide diphosphatases and are likely to have roles in regulating UDP/GDP concentrations in the Golgi lumen. C1 [Chiu, Tsan-Yu; Clark, Greg; Roux, Stanley J.] Univ Texas Austin, Sect Mol Cell & Dev Biol, Austin, TX 78712 USA. [Christiansen, Katy; Lao, Jeemeng; Loque, Dominique; Heazlewood, Joshua L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint BioEnergy Inst, Berkeley, CA 94720 USA. [Christiansen, Katy; Lao, Jeemeng; Loque, Dominique; Heazlewood, Joshua L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Moreno, Ignacio; Orellana, Ariel] Univ Andres Bello, Ctr Biotecnol Vegetal, FONDAP Ctr Genome Regulat, Santiago 8370146, RM, Chile. RP Roux, SJ (reprint author), Univ Texas Austin, Sect Mol Cell & Dev Biol, Austin, TX 78712 USA. EM sroux@uts.cc.utexas.edu RI Heazlewood, Joshua/A-2554-2008; Loque, Dominique/A-8153-2008; Orellana, Ariel/E-2166-2014 OI Heazlewood, Joshua/0000-0002-2080-3826; Orellana, Ariel/0000-0002-9243-808X FU National Science Foundation [0718890, 1027514]; FONDECYT [1110954, ICM-P10-062-F, Basal Program PFB-16, FONDAP-CRG]; Office of Science, Office of Biological and Environmental Research, of the US Department of Energy [DE-AC02-05CH11231] FX This study was supported by the National Science Foundation [grant Nos. 0718890 and 1027514 (to S.J.R. and G. B. C)]; FONDECYT 1110954, ICM-P10-062-F, Basal Program PFB-16, FONDAP-CRG [to A.O.]. The work conducted by the Joint BioEnergy Institute was supported by the Office of Science, Office of Biological and Environmental Research, of the US Department of Energy under Contract No. DE-AC02-05CH11231. NR 64 TC 15 Z9 16 U1 1 U2 19 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0032-0781 J9 PLANT CELL PHYSIOL JI Plant Cell Physiol. PD NOV PY 2012 VL 53 IS 11 BP 1913 EP 1925 DI 10.1093/pcp/pcs131 PG 13 WC Plant Sciences; Cell Biology SC Plant Sciences; Cell Biology GA 034SE UT WOS:000310892400008 PM 23034877 ER PT J AU Schwender, J Hay, JO AF Schwender, Joerg Hay, Jordan O. TI Predictive Modeling of Biomass Component Tradeoffs in Brassica napus Developing Oilseeds Based on in Silico Manipulation of Storage Metabolism SO PLANT PHYSIOLOGY LA English DT Article ID PYRUVATE-DEHYDROGENASE KINASE; SEED OIL CONTENT; FLUX VARIABILITY ANALYSIS; ERUCIC-ACID CONTENT; PLANT-CELLS; INORGANIC PYROPHOSPHATE; ARABIDOPSIS-THALIANA; CHLAMYDOMONAS-REINHARDTII; NETWORK RECONSTRUCTION; STOICHIOMETRIC MODEL AB Seed oil content is a key agronomical trait, while the control of carbon allocation into different seed storage compounds is still poorly understood and hard to manipulate. Using bna572, a large-scale model of cellular metabolism in developing embryos of rapeseed (Brassica napus) oilseeds, we present an in silico approach for the analysis of carbon allocation into seed storage products. Optimal metabolic flux states were obtained by flux variability analysis based on minimization of the uptakes of substrates in the natural environment of the embryo. For a typical embryo biomass composition, flux sensitivities to changes in different storage components were derived. Upper and lower flux bounds of each reaction were categorized as oil or protein responsive. Among the most oil-responsive reactions were glycolytic reactions, while reactions related to mitochondrial ATP production were most protein responsive. To assess different biomass compositions, a tradeoff between the fractions of oil and protein was simulated. Based on flux-bound discontinuities and shadow prices along the tradeoff, three main metabolic phases with distinct pathway usage were identified. Transitions between the phases can be related to changing modes of the tricarboxylic acid cycle, reorganizing the usage of organic carbon and nitrogen sources for protein synthesis and acetylcoenzyme A for cytosol-localized fatty acid elongation. The phase close to equal oil and protein fractions included an unexpected pathway bypassing a-ketoglutarate-oxidizing steps in the tricarboxylic acid cycle. The in vivo relevance of the findings is discussed based on literature on seed storage metabolism. C1 [Schwender, Joerg; Hay, Jordan O.] Brookhaven Natl Lab, Dept Biol, Upton, NY 11973 USA. RP Schwender, J (reprint author), Brookhaven Natl Lab, Dept Biol, Upton, NY 11973 USA. EM schwend@bnl.gov RI Schwender, Jorg/P-2282-2014 OI Schwender, Jorg/0000-0003-1350-4171 FU U.S. Department of Energy, Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences [BO-133] FX This work was supported by the U.S. Department of Energy, Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences (field work proposal no. BO-133). NR 87 TC 22 Z9 22 U1 0 U2 25 PU AMER SOC PLANT BIOLOGISTS PI ROCKVILLE PA 15501 MONONA DRIVE, ROCKVILLE, MD 20855 USA SN 0032-0889 J9 PLANT PHYSIOL JI Plant Physiol. PD NOV PY 2012 VL 160 IS 3 BP 1218 EP 1236 DI 10.1104/pp.112.203927 PG 19 WC Plant Sciences SC Plant Sciences GA 030QC UT WOS:000310584200007 PM 22984123 ER PT J AU Cao, B Zweben, SJ Stotler, DP Bell, M Diallo, A Kaye, SM LeBlanc, B AF Cao, B. Zweben, S. J. Stotler, D. P. Bell, M. Diallo, A. Kaye, S. M. LeBlanc, B. TI Edge turbulence velocity changes with lithium coating on NSTX SO PLASMA PHYSICS AND CONTROLLED FUSION LA English DT Article ID DIII-D TOKAMAK; NEUTRALS; TRANSITION; THRESHOLD; PLASMAS AB Lithium coating improves energy confinement and eliminates edge-localized modes in the National Spherical Torus Experiment (NSTX), but the mechanism of this improvement is not yet well understood. We used the gas-puff-imaging diagnostic on NSTX to measure the changes in edge turbulence which occurred during a scan with variable lithium wall coating, in order to help understand the reason for the confinement improvement with lithium. There was a small increase in the edge turbulence poloidal velocity and a decrease in the poloidal velocity fluctuation level with increased lithium. The possible effect of varying edge neutral density on turbulence damping was evaluated for these cases in NSTX. C1 [Cao, B.] Chinese Acad Sci, Inst Plasma Phys, Hefei 230031, Peoples R China. [Zweben, S. J.; Stotler, D. P.; Bell, M.; Diallo, A.; Kaye, S. M.; LeBlanc, B.] Princeton Plasma Phys Lab, Princeton, NJ 08540 USA. RP Cao, B (reprint author), Chinese Acad Sci, Inst Plasma Phys, Hefei 230031, Peoples R China. RI Stotler, Daren/J-9494-2015 OI Stotler, Daren/0000-0001-5521-8718 FU National Nature Science Foundation of China [11021565]; US DOE [DE-AC02-09CH11466] FX The authors wish to thank B LaBombard of MIT and B Davis of PPPL for the help with KN1D, R J Maqueda for taking the GPI data used in this experiment, F Scotti of PPPL for the help with the calibration of the GPI camera, V Soukanovskii and F Scotti for divertor data and R J Maqueda, R Maingi, J M Canik and W X Wang for very helpful comments. One of us (Bin Cao) thanks the NSTX team for support during his visit to PPPL. This research was funded by the National Nature Science Foundation of China under Contract No 11021565 and US DOE Contract DE-AC02-09CH11466. NR 24 TC 5 Z9 5 U1 8 U2 12 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0741-3335 J9 PLASMA PHYS CONTR F JI Plasma Phys. Control. Fusion PD NOV PY 2012 VL 54 IS 11 AR 112001 DI 10.1088/0741-3335/54/11/112001 PG 5 WC Physics, Fluids & Plasmas SC Physics GA 030HT UT WOS:000310562500001 ER PT J AU Hooper, EB Bulmer, RH Cohen, BI Hill, DN Holcomb, CT Hudson, B McLean, HS Pearlstein, LD Romero-Talamas, CA Sovinec, CR Stallard, BW Wood, RD Woodruff, S AF Hooper, E. B. Bulmer, R. H. Cohen, B. I. Hill, D. N. Holcomb, C. T. Hudson, B. McLean, H. S. Pearlstein, L. D. Romero-Talamas, C. A. Sovinec, C. R. Stallard, B. W. Wood, R. D. Woodruff, S. TI Sustained Spheromak Physics Experiment (SSPX): design and physics results SO PLASMA PHYSICS AND CONTROLLED FUSION LA English DT Review ID COAXIAL HELICITY INJECTION; MAGNETIC HELICITY; ENERGY CONFINEMENT; DRIVEN SPHEROMAK; SPHEX SPHEROMAK; PLASMA CONFIGURATION; TOROIDAL PLASMA; CTX SPHEROMAK; GUN-DRIVEN; RELAXATION AB The Sustained Spheromak Physics Experiment (SSPX) was a high-temperature (T-e up to 0.5 keV) spheromak formed by coaxial helicity injection (CHI) and with plasma duration of a few milliseconds following the high-current formation stage. Clean walls and low impurity operation were obtained by a combination of baking, discharge cleaning and titanium deposition on the walls, allowing the generation of high-quality plasmas. Resistive-magnetohydrodynamic simulations, benchmarked to the experiment, were used to elucidate the physics. The detailed characteristics of the n(phi) = 1 toroidal mode associated with CHI were determined as was the physics of the nonlinear current drive and magnetic reconnection that formed and sustained the spheromak. If the helicity injection rate was reduced following formation the plasma became relatively quiescent and magnetic surfaces formed. The measured thermal diffusivity in the core was as low as similar to 1 m(2) s(-1). However, reconnection events during buildup or sustainment of the plasma current by CHI were found to open magnetic surfaces throughout the plasma allowing rapid energy loss to the walls. As a result, experiments and simulations in SSPX found no path to simultaneous sustainment by CHI and good energy confinement. Additional physics results are also presented in this review. C1 [Hooper, E. B.; Bulmer, R. H.; Cohen, B. I.; Hill, D. N.; Holcomb, C. T.; McLean, H. S.; Pearlstein, L. D.; Stallard, B. W.; Wood, R. D.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Hudson, B.] Univ Calif San Diego, Energy Res Ctr, La Jolla, CA 92093 USA. [Romero-Talamas, C. A.] Univ Maryland, Inst Res Elect & Appl Phys, College Pk, MD 20742 USA. [Sovinec, C. R.] Univ Wisconsin, Dept Engn Phys, Madison, WI 53706 USA. [Woodruff, S.] Woodruff Sci Inc, Seattle, WA 98107 USA. RP Hooper, EB (reprint author), Lawrence Livermore Natl Lab, POB 808, Livermore, CA 94550 USA. EM hooper1@llnl.gov FU US Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; University of Wisconsin-Madison [FG02-01ER54661] FX This work was performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344, and by the University of Wisconsin-Madison under Grant No FG02-01ER54661. NR 78 TC 12 Z9 12 U1 4 U2 19 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0741-3335 J9 PLASMA PHYS CONTR F JI Plasma Phys. Control. Fusion PD NOV PY 2012 VL 54 IS 11 AR 113001 DI 10.1088/0741-3335/54/11/113001 PG 26 WC Physics, Fluids & Plasmas SC Physics GA 030HT UT WOS:000310562500002 ER PT J AU Meruelo, AD Han, SK Kim, S Bowie, JU AF Meruelo, Alejandro D. Han, Seong Kyu Kim, Sanguk Bowie, James U. TI Structural differences between thermophilic and mesophilic membrane proteins SO PROTEIN SCIENCE LA English DT Article DE stability; folding; structure; transmembrane helix; hydrogen bonds; polar amino acids; burial; kink; packing ID HELIX-HELIX INTERACTIONS; THERMAL-STABILITY; HYDROGEN-BONDS; TRANSMEMBRANE HELICES; ALPHA-HELICES; THERMOSTABILITY; PACKING; STABILIZATION; RECOGNITION; PEPTIDES AB The evolutionary adaptations of thermophilic water-soluble proteins required for maintaining stability at high temperature have been extensively investigated. Little is known about the adaptations in membrane proteins, however. Here, we compare many properties of mesophilic and thermophilic membrane protein structures, including side-chain burial, packing, hydrogen bonding, transmembrane kinks, loop lengths, hydrophobicity, and other sequence features. Most of these properties are quite similar between mesophiles and thermophiles although we observe a slight increase in side-chain burial and possibly a slight decrease in the frequency of transmembrane kinks in thermophilic membrane protein structures. The most striking difference is the increased hydrophobicity of thermophilic transmembrane helices, possibly reflecting more stringent hydrophobicity requirements for membrane partitioning at high temperature. In agreement with prior work examining transmembrane sequences, we find that thermophiles have an increase in small residues (Gly, Ala, Ser, and Val) and a strong suppression of Cys. We also find a relative dearth of most strongly polar residues (Asp, Asn, Glu, Gln, and Arg). These results suggest that in thermophiles, there is significant evolutionary pressure to offload destabilizing polar amino acids, to decrease the entropy cost of side chain burial, and to eliminate thermally sensitive amino acids. C1 [Bowie, James U.] Univ Calif Los Angeles, Dept Chem & Biochem, Inst Mol Biol, UCLA DOE Inst Genom & Prote, Los Angeles, CA 90095 USA. [Meruelo, Alejandro D.] Univ Calif Los Angeles, Med Scientist Training Program, Inst Mol Biol, UCLA DOE Inst Genom & Prote, Los Angeles, CA 90095 USA. [Han, Seong Kyu; Kim, Sanguk] Pohang Univ Sci & Technol, Div Mol & Life Sci, Pohang, South Korea. RP Bowie, JU (reprint author), Univ Calif Los Angeles, Dept Chem & Biochem, Inst Mol Biol, UCLA DOE Inst Genom & Prote, Los Angeles, CA 90095 USA. EM bowie@mbi.ucla.edu RI Meruelo, Alejandro/L-3118-2016 OI Meruelo, Alejandro/0000-0001-6087-1818 FU NIH [RO1 GM063919]; Ruth L. Kirschstein NRSA Predoctoral Fellowship Award FX Grant sponsors: NIH Grant RO1 GM063919, The Ruth L. Kirschstein NRSA Predoctoral Fellowship Award. NR 45 TC 12 Z9 12 U1 0 U2 34 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0961-8368 J9 PROTEIN SCI JI Protein Sci. PD NOV PY 2012 VL 21 IS 11 BP 1746 EP 1753 DI 10.1002/pro.2157 PG 8 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA 023KY UT WOS:000310032900014 PM 23001966 ER PT J AU Min, AB Miallau, L Sawaya, MR Habel, J Cascio, D Eisenberg, D AF Min, Andrew B. Miallau, Linda Sawaya, Michael R. Habel, Jeff Cascio, Duilio Eisenberg, David TI The crystal structure of the Rv0301-Rv0300 VapBC-3 toxin-antitoxin complex from M. tuberculosis reveals a Mg2+ ion in the active site and a putative RNA-binding site SO PROTEIN SCIENCE LA English DT Article DE tuberculosis; toxin-antitoxin; toxin; antitoxin; vapBC; vapB; vapC; protein complex; Rv0301; Rv0300; PIN-domain ID ESCHERICHIA-COLI; MYCOBACTERIUM-TUBERCULOSIS; YEFM ANTITOXIN; PIN-DOMAIN; PROTEIN; DNA; INTERFERASE; COMPLEMENTARITY; RIBONUCLEASE; TRANSLATION AB VapBC pairs account for 45 out of 88 identified toxin-antitoxin (TA) pairs in the Mycobacterium tuberculosis (Mtb) H37Rv genome. A working model suggests that under times of stress, antitoxin molecules are degraded, releasing the toxins to slow the metabolism of the cell, which in the case of VapC toxins is via their RNase activity. Otherwise the TA pairs remain bound to their promoters, autoinhibiting transcription. The crystal structure of Rv0301-Rv0300, an Mtb VapBC TA complex determined at 1.49 angstrom resolution, suggests a mechanism for these three functions: RNase activity, its inhibition by antitoxin, and its ability to bind promoter DNA. The Rv0301 toxin consists of a core of five parallel beta strands flanked by alpha helices. Three proximal aspartates coordinate a Mg2+ ion forming the putative RNase active site. The Rv0300 antitoxin monomer is extended in structure, consisting of an N-terminal beta strand followed by four helices. The last two helices wrap around the toxin and terminate near the putative RNase active site, but with different conformations. In one conformation, the C-terminal arginine interferes with Mg2+ ion coordination, suggesting a mechanism by which the antitoxin can inhibit toxin activity. At the N-terminus of the antitoxin, two pairs of Ribbon-Helix-Helix (RHH) motifs are related by crystallographic twofold symmetry. The resulting hetero-octameric complex is similar to the FitAB system, but the two RHH motifs are about 30 angstrom closer together in the Rv0301-Rv0300 complex, suggesting either a different span of the DNA recognition sequence or a conformational change. C1 [Min, Andrew B.; Miallau, Linda; Sawaya, Michael R.; Cascio, Duilio; Eisenberg, David] Univ Calif Los Angeles, Dept Chem & Biochem, Howard Hughes Med Inst, UCLA Inst Genom & Prote, Los Angeles, CA 90095 USA. [Habel, Jeff] Univ Calif Berkeley, EO Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Eisenberg, D (reprint author), Univ Calif Los Angeles, Dept Chem & Biochem, Howard Hughes Med Inst, UCLA Inst Genom & Prote, Box 951570, Los Angeles, CA 90095 USA. EM david@mbi.ucla.edu OI Sawaya, Michael/0000-0003-0874-9043 FU National Science Foundation [MCB-0958111]; National Institutes of Health [A1068135-04]; U.S. Department of Energy [DE-FC02-02ER63421]; DOE [DE-FC02-02ER63421, DE-AC02-06CH11357]; National Center for Research Resources [5P41RR015301-10]; National Institute of General Medical Sciences from the National Institutes of Health [8 P41 GM103403-10] FX Grant sponsor: National Science Foundation; Grant number: MCB-0958111; Grant sponsor: National Institutes of Health; Grant number: A1068135-04; Grant sponsor: U.S. Department of Energy; Grant number: DE-FC02-02ER63421.; The authors thank Janet Chiang for the initial construct, and Dr. Mark Arbing and Dr. Arthur Laganowsky for many helpful discussions. They also thank the UCLA-DOE X-ray Crystallography Core Facility, which is supported by DOE Grant DE-FC02-02ER63421; M. Capel, K. Rajashankar, N. Sukumar, J. Schuermann, I. Kourinov and F. Murphy at NECAT beamlines 24-ID at APS, which are supported by grants from the National Center for Research Resources (5P41RR015301-10), and the National Institute of General Medical Sciences (8 P41 GM103403-10) from the National Institutes of Health. Use of the APS is supported by DOE under Contract DE-AC02-06CH11357. NR 47 TC 23 Z9 27 U1 0 U2 5 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0961-8368 J9 PROTEIN SCI JI Protein Sci. PD NOV PY 2012 VL 21 IS 11 BP 1754 EP 1767 DI 10.1002/pro.2161 PG 14 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA 023KY UT WOS:000310032900015 PM 23011806 ER PT J AU Hengel, SM Floyd, E Baker, ES Zhao, R Wu, S Pasa-Tolic, L AF Hengel, Shawna M. Floyd, Erica Baker, Erin S. Zhao, Rui Wu, Si Pasa-Tolic, Ljiljana TI Evaluation of SDS depletion using an affinity spin column and IMS-MS detection SO PROTEOMICS LA English DT Article DE Detergents; Ion mobility; Sample preparation; SDS depletion; Technology ID ION MOBILITY SPECTROMETRY; SODIUM DODECYL-SULFATE; BIOCHEMICAL SAMPLES; MASS-SPECTROMETRY; PROTEOME ANALYSIS; SEPARATION; QUANTIFICATION; DETERGENTS; PEPTIDES AB While the use of detergents is necessary for a variety of protein isolation preparation protocols, they are not compatible with mass spectral analysis due to ion suppression and adduct formation. This manuscript describes optimization of detergent removal, using commercially available SDS depletion spin columns containing an affinity resin, providing for both increased protein recovery and thorough SDS removal. Ion mobility spectrometry coupled with mass spectrometry (IMS-MS) allowed for a concurrent analysis of both analyte and detergent. In the case of both proteins and peptides, higher detergent concentrations than previously reported provided an increase of sample recovery; however there was a limit as SDS was detected by IMS-MS at higher levels of SDS indicating incomplete detergent depletion. The results also suggest that optimal conditions for SDS removal are dependent on the sample concentration. Overall, this study provides a useful guide for proteomic studies where SDS is required for efficient sample preparation. C1 [Hengel, Shawna M.; Floyd, Erica; Zhao, Rui; Wu, Si; Pasa-Tolic, Ljiljana] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Baker, Erin S.] Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99352 USA. RP Pasa-Tolic, L (reprint author), Pacific NW Natl Lab, Environm Mol Sci Lab, 902 Battelle Blvd,POB 999,MSIN K8-98, Richland, WA 99352 USA. EM ljiljana.pasatolic@pnnl.gov FU US Department of Energy (DOE) Office of Biological and Environmental Research; NIH National Center for Research Resources [RR018522]; DOE/BER Genomics: Genome Sciences program; NIGMS [P41 GM103493]; DOE [DE-AC05-76RLO 1830] FX This research was supported by the US Department of Energy (DOE) Office of Biological and Environmental Research and by the NIH National Center for Research Resources (RR018522), DOE/BER Genomics: Genome Sciences program and NIGMS (P41 GM103493). Work was performed in the Environmental Molecular Science Laboratory (EMSL), a DOE national scientific user facility located on the campus of Pacific Northwest National Laboratory (PNNL) in Richland, Washington. PNNL is a multiprogram national laboratory operated by Battelle for the DOE under Contract DE-AC05-76RLO 1830. The authors also wish to thank Carrie Nicora and Heather Brewer for insightful discussion. NR 13 TC 12 Z9 13 U1 0 U2 12 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1615-9853 J9 PROTEOMICS JI Proteomics PD NOV PY 2012 VL 12 IS 21 BP 3138 EP 3142 DI 10.1002/pmic.201200168 PG 5 WC Biochemical Research Methods; Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA 030IJ UT WOS:000310564100003 PM 22936678 ER PT J AU Bloom, JS Richards, JW Nugent, PE Quimby, RM Kasliwal, MM Starr, DL Poznanski, D Ofek, EO Cenko, SB Butler, NR Kulkarni, SR Gal-Yam, A Law, N AF Bloom, J. S. Richards, J. W. Nugent, P. E. Quimby, R. M. Kasliwal, M. M. Starr, D. L. Poznanski, D. Ofek, E. O. Cenko, S. B. Butler, N. R. Kulkarni, S. R. Gal-Yam, A. Law, N. TI Automating Discovery and Classification of Transients and Variable Stars in the Synoptic Survey Era SO PUBLICATIONS OF THE ASTRONOMICAL SOCIETY OF THE PACIFIC LA English DT Article ID DIGITAL SKY SURVEY; SUPERNOVA SN 2011FE; SUPERVISED CLASSIFICATION; IA SUPERNOVA; TELESCOPE; PROGENITOR; GALAXY; SELECTION; DATABASE AB The rate of image acquisition in modern synoptic imaging surveys has already begun to outpace the feasibility of keeping astronomers in the real-time discovery and classification loop. Here we present the inner workings of a framework, based on machine-learning algorithms, that captures expert training and ground-truth knowledge about the variable and transient sky to automate (1) the process of discovery on image differences, and (2) the generation of preliminary science-type classifications of discovered sources. Since follow-up resources for extracting novel science from fast-changing transients are precious, self-calibrating classification probabilities must be couched in terms of efficiencies for discovery and purity of the samples generated. We estimate the purity and efficiency in identifying real sources with a two-epoch image-difference discovery algorithm for the Palomar Transient Factory (PTF) survey. Once given a source discovery, using machine-learned classification trained on PTF data, we distinguish between transients and variable stars with a 3.8% overall error rate (with 1.7% errors for imaging within the Sloan Digital Sky Survey footprint). At >96% classification efficiency, the samples achieve 90% purity. Initial classifications are shown to rely primarily on context-based features, determined from the data itself and external archival databases. In the first year of autonomous operations of PTF, this discovery and classification framework led to several significant science results, from outbursting young stars to subluminous Type IIP supernovae to candidate tidal disruption events. We discuss future directions of this approach, including the possible roles of crowdsourcing and the scalability of machine learning to future surveys such as the Large Synoptic Survey Telescope (LSST). C1 [Bloom, J. S.; Richards, J. W.; Nugent, P. E.; Starr, D. L.; Poznanski, D.; Cenko, S. B.; Butler, N. R.] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. [Bloom, J. S.; Nugent, P. E.; Poznanski, D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Richards, J. W.] Univ Calif Berkeley, Dept Stat, Berkeley, CA 94720 USA. [Quimby, R. M.; Kasliwal, M. M.; Ofek, E. O.; Kulkarni, S. R.] CALTECH, Cahill Ctr Astrophys, Pasadena, CA 91125 USA. [Quimby, R. M.] Univ Tokyo, IPMU, Kashiwa, Chiba 2778583, Japan. [Kasliwal, M. M.] Observ Carnegie Inst Sci, Pasadena, CA 91101 USA. [Poznanski, D.] Tel Aviv Univ, Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Ofek, E. O.; Gal-Yam, A.] Weizmann Inst Sci, Dept Particle Phys & Astrophys, Fac Phys, IL-76100 Rehovot, Israel. [Butler, N. R.] Arizona State Univ, Sch Earth & Space Explorat, Tempe, AZ 85287 USA. [Law, N.] Univ Toronto, Dunlap Inst Astron & Astrophys, Toronto, ON M5S 3H4, Canada. RP Bloom, JS (reprint author), Univ Calif Berkeley, Dept Astron, 601 Campbell Hall, Berkeley, CA 94720 USA. FU National Science Foundation [0941742, 0908886]; National Aeronautics and Space Administration (NASA) [NNX10AI21G, NNX1OA057G]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; W.M. Keck Foundation FX The authors acknowledge the generous support of a CDI grant (#0941742) from the National Science Foundation. J.S.B. and D. L. S. also thank the Las Cumbres Observatory for support during the early stages of this work. S. B. C. wishes to acknowledge generous support from Gary and Cynthia Bengier, the Richard and Rhoda Goldman Fund, National Aeronautics and Space Administration (NASA)/Swift grant NNX10AI21G, NASA/Fermi grant NNX1OA057G, and National Science Foundation (NSF) grant AST-0908886. The National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract #DE-AC02-05CH11231, provided staff, computational resources, and data storage for this project.; Some of the data presented herein were obtained at the W.M. Keck Observatory, which is operated as a scientific partnership among the California Institute of Technology, the University of California, and the National Aeronautics and Space Administration. The Observatory was made possible by the generous financial support of the W.M. Keck Foundation. The authors wish to recognize and acknowledge the very significant cultural role and reverence that the summit of Mauna Kea has always had within the indigenous Hawaiian community. We are most fortunate to have the opportunity to conduct observations from this mountain. This research has made use of the VizieR catalogue access tool, CDS, Strasbourg, France (Ochsenbein et al. 2000). NR 61 TC 47 Z9 47 U1 3 U2 10 PU UNIV CHICAGO PRESS PI CHICAGO PA 1427 E 60TH ST, CHICAGO, IL 60637-2954 USA SN 0004-6280 J9 PUBL ASTRON SOC PAC JI Publ. Astron. Soc. Pac. PD NOV PY 2012 VL 124 IS 921 BP 1175 EP 1196 DI 10.1086/668468 PG 22 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 035AO UT WOS:000310914200004 ER PT J AU Zhang, KW Zeng, FW Wang, H Lin, HT AF Zhang, Kewei Zeng, Fan Wen Wang, Hong Lin, Hua-Tay TI Strength properties of aged poled lead zirconate titanate subjected to electromechanical loadings SO SMART MATERIALS AND STRUCTURES LA English DT Article ID FATIGUE-CRACK GROWTH; ELECTRIC-FIELD; BIAXIAL FLEXURE; PZT CERAMICS; BEHAVIOR AB Electric field and aging time are two important factors that affect the mechanical strength and long-term reliability of lead zirconate titanate or PZT actuators. In the present work, a commercial PZT-5A aged four years was examined using ball-on-ring (BoR) mechanical testing under coupled electric fields. The electric field range of -3E(c) to +3E(c) (E-c, coercive electric field) was studied (i.e., -3E(c), -E-c, 0, +E-c, +2E(c), and +3E(c)) with a controlled electric loading path. A Weibull distribution was used to interpret the mechanical strength data. With an electric field preloaded from 0 to -3E(c), it was found that subsequent increases in the electric field resulted in an asymmetrical V-shaped curve of mechanical strength against the electric field. The bottom of the V curve was located near the zero electric field level. Microscopy analysis showed that pores were the strength limiter for the tested PZT under electromechanical loadings. C1 [Zhang, Kewei; Zeng, Fan Wen; Wang, Hong; Lin, Hua-Tay] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Zhang, KW (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. EM wangh@ornl.gov RI Wang, Hong/O-1987-2016 OI Wang, Hong/0000-0002-0173-0545 FU US Department of Energy [DE-AC05-00OR22725]; UT-Battelle, LLC FX Research was sponsored by the US Department of Energy, Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies, as part of the Propulsion Materials Program, under contract DE-AC05-00OR22725 with UT-Battelle, LLC. The authors are grateful to Drs Andrew A Wereszczak and Fei Ren for reviewing the manuscript and giving helpful suggestions. NR 22 TC 1 Z9 1 U1 1 U2 12 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0964-1726 J9 SMART MATER STRUCT JI Smart Mater. Struct. PD NOV PY 2012 VL 21 IS 11 AR 117001 DI 10.1088/0964-1726/21/11/117001 PG 7 WC Instruments & Instrumentation; Materials Science, Multidisciplinary SC Instruments & Instrumentation; Materials Science GA 030DC UT WOS:000310547900035 ER PT J AU Stull, CJ Hemez, FM Farrar, CR AF Stull, Christopher J. Hemez, Francois M. Farrar, Charles R. TI On assessing the robustness of structural health monitoring technologies SO STRUCTURAL HEALTH MONITORING-AN INTERNATIONAL JOURNAL LA English DT Article DE Structural health monitoring; information-gap decision theory; decision making; model selection; uncertainty; autoregressive model ID DAMAGE DETECTION; MODEL SELECTION; ROC CURVE; IDENTIFICATION; ALGORITHMS; AREA AB As structural health monitoring continues to gain popularity, both as an area of research and as a tool for use in industrial applications, the number of technologies associated with structural health monitoring will also continue to grow. As a result, the engineer tasked with developing a structural health monitoring system is faced with myriad hardware and software technologies from which to choose, often adopting an ad hoc qualitative approach based on physical intuition or past experience to making such decisions, and offering little in the way of justification for a particular decision. This article offers a framework that aims to provide the engineer with a quantitative approach for choosing from among a suite of candidate structural health monitoring technologies. The framework is outlined for the general case, where a supervised learning approach to structural health monitoring is adopted and is then demonstrated on two problems commonly encountered when developing structural health monitoring systems: (a) selection of damage-sensitive features, where the engineer must determine the appropriate order of an autoregressive model for modeling of time-history data, and (b) selection of a damage classifier, where the engineer must select from among a suite of candidate classifiers, the one most appropriate for the task at hand. The data employed for these problems are taken from a preliminary study that examined the feasibility of applying structural health monitoring technologies to the RAPid Telescopes for Optical Response observatory network. C1 [Stull, Christopher J.; Hemez, Francois M.; Farrar, Charles R.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Stull, CJ (reprint author), Los Alamos Natl Lab, POB 1663,MS P915, Los Alamos, NM 87545 USA. EM stull@lanl.gov OI Farrar, Charles/0000-0001-6533-6996; Hemez, Francois/0000-0002-5319-4078 FU National Nuclear Security Administration of the U.S. Department of Energy [DE-AC52-06NA25396] FX Los Alamos National Laboratory, an affirmative action/equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy under contract DE-AC52-06NA25396. NR 20 TC 7 Z9 7 U1 1 U2 14 PU SAGE PUBLICATIONS LTD PI LONDON PA 1 OLIVERS YARD, 55 CITY ROAD, LONDON EC1Y 1SP, ENGLAND SN 1475-9217 EI 1741-3168 J9 STRUCT HEALTH MONIT JI Struct. Health Monit. PD NOV PY 2012 VL 11 IS 6 BP 712 EP 723 DI 10.1177/1475921712451956 PG 12 WC Engineering, Multidisciplinary; Instruments & Instrumentation SC Engineering; Instruments & Instrumentation GA 032TH UT WOS:000310741500007 ER PT J AU Michalak, WD Miller, JB Yolcu, C Gellman, AJ AF Michalak, William D. Miller, James B. Yolcu, Cem Gellman, Andrew J. TI Fabrication of metallic nanoparticles by spinodal dewetting of thin films: A high-throughput approach SO THIN SOLID FILMS LA English DT Article DE Spinodal dewetting; Metal nanoparticles; High-throughput; Structural gradient; Thin films; Palladium; Silicon nitride ID LIQUID-FILMS; SPONTANEOUS RUPTURE; CONTACT ANGLES; INSTABILITY; SURFACE; FORCES; CATALYST; SIZE AB Metal nanoparticles on structured supports are used in a variety of technological applications including biosensing, energy harvesting, and electronics. In every case, the functions and properties of the metallic nanostructures depend on both their composition and structure (i.e. size, shape, and spatial distribution). Among the challenges to the development of metal nanoparticles for these applications is the characterization of relationships between their structure and their functional properties over multiple structural degrees of freedom spanning a large range of values. In this work, a method for creating a morphological gradient of metal nanoparticles on a substrate is described. The approach, suited for high-throughput fabrication and characterization, is based on spinodal dewetting of a metallic thin film from its substrate. Through control of initial film thickness, anneal temperature, and anneal time, spinodal dewetting results in supported nanoparticles with well-defined and controlled structure. The approach is demonstrated through its application to preparation of Pd nanoparticles on a silicon nitride substrate. The morphologies of the particles were characterized by scanning electron and atomic force microscopies. Free energy-based stability and topological analyses were used to confirm the dewetting mechanism. In addition, the stability theory provides a connection to the thermophysical properties of the resulting nanoparticle array. The dewetting approach is general to any metal/support system and provides an alternative, inexpensive, and robust means to rapidly create metal nanostructures with control of morphology. It shows promise for large scale production of metal nanoparticles structures, as well as understanding basic stability properties of thin metal films. (C) 2012 Elsevier B.V. All rights reserved. C1 [Michalak, William D.; Miller, James B.; Gellman, Andrew J.] US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15262 USA. [Michalak, William D.; Miller, James B.; Gellman, Andrew J.] Carnegie Mellon Univ, Dept Chem Engn, Pittsburgh, PA 15213 USA. [Yolcu, Cem] Carnegie Mellon Univ, Dept Phys, Pittsburgh, PA 15213 USA. RP Gellman, AJ (reprint author), US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15262 USA. EM gellman@cmu.edu RI Gellman, Andrew/M-2487-2014; OI Gellman, Andrew/0000-0001-6618-7427; Yolcu, Cem/0000-0002-0722-9161 NR 48 TC 5 Z9 5 U1 2 U2 41 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0040-6090 J9 THIN SOLID FILMS JI Thin Solid Films PD NOV 1 PY 2012 VL 522 BP 473 EP 479 DI 10.1016/j.tsf.2012.07.041 PG 7 WC Materials Science, Multidisciplinary; Materials Science, Coatings & Films; Physics, Applied; Physics, Condensed Matter SC Materials Science; Physics GA 033GK UT WOS:000310782000085 ER PT J AU Siddens, LK Larkin, A Krueger, SK Bradfield, CA Waters, KM Tilton, SC Pereira, CB Lohr, CV Arlt, VM Phillips, DH Williams, DE Baird, WM AF Siddens, Lisbeth K. Larkin, Andrew Krueger, Sharon K. Bradfield, Christopher A. Waters, Katrina M. Tilton, Susan C. Pereira, Cliff B. Loehr, Christiane V. Arlt, Volker M. Phillips, David H. Williams, David E. Baird, William M. TI Polycyclic aromatic hydrocarbons as skin carcinogens: Comparison of benzo [a]pyrene, dibenzo[def,p]chrysene and three environmental mixtures in the FVB/N mouse SO TOXICOLOGY AND APPLIED PHARMACOLOGY LA English DT Article DE PAHs; Cyp1a1; Cyp1b1; Adducts; Relative potency factor; Skin ID STANDARDIZED COMPLEX MIXTURE; TUMOR-INITIATING ACTIVITY; SQUAMOUS-CELL CARCINOMAS; LUNG-CANCER RISK; METABOLIC-ACTIVATION; DNA-ADDUCTS; COAL-TAR; TRANSPLACENTAL CARCINOGENESIS; CYTOCHROME-P450 1B1; TRANS-DIHYDRODIOLS AB The polycyclic aromatic hydrocarbon (PAH), benzo[a]pyrene (BaP), was compared to dibenzo[def,p]chrysene (DBC) and combinations of three environmental PAH mixtures (coal tar, diesel particulate and cigarette smoke condensate) using a two stage, FVB/N mouse skin tumor model. DBC (4 nmol) was most potent, reaching 100% tumor incidence with a shorter latency to tumor formation, less than 20 weeks of 12-O-tetradecanoylphorbol-13-acetate (TPA) promotion compared to all other treatments. Multiplicity was 4 times greater than BaP (400 nmol). Both PAHs produced primarily papillomas followed by squamous cell carcinoma and carcinoma in situ. Diesel particulate extract (1 mg SRM 1650b; mix 1) did not differ from toluene controls and failed to elicit a carcinogenic response. Addition of coal tar extract (1 mg SRM 1597a; mix 2) produced a response similar to BaP. Further addition of 2 mg of cigarette smoke condensate (mix 3) did not alter the response with mix 2. PAH-DNA adducts measured in epidermis 12 h post initiation and analyzed by P-32 post-labeling, did not correlate with tumor incidence. PAH-dependent alteration in transcriptome of skin 12 h post initiation was assessed by microarray. Principal component analysis (sum of all treatments) of the 922 significantly altered genes (p < 0.05), showed DBC and BaP to cluster distinct from PAH mixtures and each other. BaP and mixtures up-regulated phase 1 and phase 2 metabolizing enzymes while DBC did not The carcinogenicity with DBC and two of the mixtures was much greater than would be predicted based on published Relative Potency Factors (RPFs). (c) 2012 Elsevier Inc. All rights reserved. C1 [Siddens, Lisbeth K.; Larkin, Andrew; Krueger, Sharon K.; Waters, Katrina M.; Tilton, Susan C.; Pereira, Cliff B.; Williams, David E.; Baird, William M.] Oregon State Univ, Superfund Res Ctr, Corvallis, OR 97331 USA. [Siddens, Lisbeth K.; Larkin, Andrew; Williams, David E.; Baird, William M.] Oregon State Univ, Dept Environm & Mol Toxicol, Corvallis, OR 97331 USA. [Krueger, Sharon K.; Williams, David E.] Oregon State Univ, Linus Pauling Inst, Corvallis, OR 97331 USA. [Bradfield, Christopher A.] Univ Wisconsin, McArdle Lab Canc Res, Madison, WI 53706 USA. [Waters, Katrina M.; Tilton, Susan C.] Pacific NW Natl Lab, Computat Biol & Bioinformat Grp, Richland, WA 99352 USA. [Pereira, Cliff B.] Oregon State Univ, Deptartment Stat, Corvallis, OR 97331 USA. [Pereira, Cliff B.; Loehr, Christiane V.; Williams, David E.; Baird, William M.] Oregon State Univ, Environm Hlth Sci Ctr, Corvallis, OR 97331 USA. [Loehr, Christiane V.] Oregon State Univ, Coll Vet Med, Corvallis, OR 97331 USA. [Arlt, Volker M.; Phillips, David H.] Kings Coll London, MRC HPA Ctr Environm & Hlth, Analyt & Environm Sci Div, London SE1 9NH, England. RP Williams, DE (reprint author), Oregon State Univ, Superfund Res Ctr, 435 Weniger Hall, Corvallis, OR 97331 USA. EM david.williams@oregonstate.edu OI Phillips, David/0000-0001-8509-3485 FU National Institute of Environmental Health [P42ES016465, P42ES016465-S1]; Cancer Research UK FX This work was supported by the National Institute of Environmental Health (grants P42ES016465 and P42ES016465-S1). Work at King's College London is supported by Cancer Research UK. NR 66 TC 36 Z9 37 U1 3 U2 29 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0041-008X EI 1096-0333 J9 TOXICOL APPL PHARM JI Toxicol. Appl. Pharmacol. PD NOV 1 PY 2012 VL 264 IS 3 BP 377 EP 386 DI 10.1016/j.taap.2012.08.014 PG 10 WC Pharmacology & Pharmacy; Toxicology SC Pharmacology & Pharmacy; Toxicology GA 031VG UT WOS:000310670000009 PM 22935520 ER PT J AU Massoudi, M Uguz, AK AF Massoudi, Mehrdad Uguz, A. K. TI Chemically-reacting fluids with variable transport properties SO APPLIED MATHEMATICS AND COMPUTATION LA English DT Article DE Non-linear fluids; Chemically-reacting fluids; Variable viscosity; Variable thermal conductivity; Variable diffusion coefficient; Viscous dissipation ID FLOWING GRANULAR-MATERIALS; HEAT-FLUX VECTOR; VISCOUS DISSIPATION; NONLINEAR FLUID; MIXTURE AB In this paper we study the flow and heat transfer in a chemically-reacting fluid, whose transport properties, i.e., viscosity, thermal conductivity and the diffusion coefficients, are assumed to be a function of the concentration. The equations for the shearing flow of such a fluid between two long horizontal parallel plates, which are at different temperatures, are made dimensionless and the boundary value problem is solved numerically; the velocity, concentration and temperature profiles are obtained for various dimensionless numbers. Published by Elsevier Inc. C1 [Massoudi, Mehrdad] US DOE, NETL, Pittsburgh, PA 15236 USA. [Uguz, A. K.] Bogazici Univ, Dept Chem Engn, TR-34342 Istanbul, Turkey. RP Massoudi, M (reprint author), US DOE, NETL, POB 10940,626 Cochrans Mill Rd, Pittsburgh, PA 15236 USA. EM MASSOUDI@NETL.DOE.GOV FU Bogazici University [6007] FX Kerem Uguz acknowledges financial support from Bogazici University Research Fund Project 6007. NR 30 TC 0 Z9 0 U1 0 U2 2 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 0096-3003 J9 APPL MATH COMPUT JI Appl. Math. Comput. PD NOV 1 PY 2012 VL 219 IS 4 BP 1761 EP 1775 DI 10.1016/j.amc.2012.08.015 PG 15 WC Mathematics, Applied SC Mathematics GA 029OB UT WOS:000310504000033 ER PT J AU Bolton, AS Schlegel, DJ Aubourg, E Bailey, S Bhardwaj, V Brownstein, JR Burles, S Chen, YM Dawson, K Eisenstein, DJ Gunn, JE Knapp, GR Loomis, CP Lupton, RH Maraston, C Muna, D Myers, AD Olmstead, MD Padmanabhan, N Paris, I Percival, WJ Petitjean, P Rockosi, CM Ross, NP Schneider, DP Shu, YP Strauss, MA Thomas, D Tremonti, CA Wake, DA Weaver, BA Wood-Vasey, WM AF Bolton, Adam S. Schlegel, David J. Aubourg, Eric Bailey, Stephen Bhardwaj, Vaishali Brownstein, Joel R. Burles, Scott Chen, Yan-Mei Dawson, Kyle Eisenstein, Daniel J. Gunn, James E. Knapp, G. R. Loomis, Craig P. Lupton, Robert H. Maraston, Claudia Muna, Demitri Myers, Adam D. Olmstead, Matthew D. Padmanabhan, Nikhil Paris, Isabelle Percival, Will J. Petitjean, Patrick Rockosi, Constance M. Ross, Nicholas P. Schneider, Donald P. Shu, Yiping Strauss, Michael A. Thomas, Daniel Tremonti, Christy A. Wake, David A. Weaver, Benjamin A. Wood-Vasey, W. Michael TI SPECTRAL CLASSIFICATION AND REDSHIFT MEASUREMENT FOR THE SDSS-III BARYON OSCILLATION SPECTROSCOPIC SURVEY SO ASTRONOMICAL JOURNAL LA English DT Article DE methods: data analysis; surveys; techniques: spectroscopic ID DIGITAL SKY SURVEY; STELLAR POPULATION-MODELS; QUASAR TARGET SELECTION; STAR-FORMING GALAXIES; LUMINOUS RED GALAXIES; DATA RELEASE; LINE SPECTRA; RESOLUTION; EMISSION; LIBRARY AB We describe the automated spectral classification, redshift determination, and parameter measurement pipeline in use for the Baryon Oscillation Spectroscopic Survey (BOSS) of the Sloan Digital Sky Survey III (SDSS-III) as of the survey's ninth data release (DR9), encompassing 831,000 moderate-resolution optical spectra. We give a review of the algorithms employed, and describe the changes to the pipeline that have been implemented for BOSS relative to previous SDSS-I/II versions, including new sets of stellar, galaxy, and quasar redshift templates. For the color-selected "CMASS" sample of massive galaxies at redshift 0.4 less than or similar to z <= 0.8 targeted by BOSS for the purposes of large-scale cosmological measurements, the pipeline achieves an automated classification success rate of 98.7% and confirms 95.4% of unique CMASS targets as galaxies (with the balance being mostly M stars). Based on visual inspections of a subset of BOSS galaxies, we find that approximately 0.2% of confidently reported CMASS sample classifications and redshifts are incorrect, and about 0.4% of all CMASS spectra are objects unclassified by the current algorithm which are potentially recoverable. The BOSS pipeline confirms that similar to 51.5% of the quasar targets have quasar spectra, with the balance mainly consisting of stars and low signal-to-noise spectra. Statistical (as opposed to systematic) redshift errors propagated from photon noise are typically a few tens of km s(-1) for both galaxies and quasars, with a significant tail to a few hundreds of km s(-1) for quasars. We test the accuracy of these statistical redshift error estimates using repeat observations, finding them underestimated by a factor of 1.19-1.34 for galaxies and by a factor of two for quasars. We assess the impact of sky-subtraction quality, signal-to-noise ratio, and other factors on galaxy redshift success. Finally, we document known issues with the BOSS DR9 spectroscopic data set and describe directions of ongoing development. C1 [Bolton, Adam S.; Brownstein, Joel R.; Dawson, Kyle; Olmstead, Matthew D.; Shu, Yiping] Univ Utah, Dept Phys & Astron, Salt Lake City, UT 84112 USA. [Schlegel, David J.; Bailey, Stephen; Ross, Nicholas P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Aubourg, Eric] Univ Paris Diderot, Astroparticule & Cosmol APC, F-75205 Paris 13, France. [Aubourg, Eric] CEA, Ctr Saclay, Irfu SPP, F-91191 Gif Sur Yvette, France. [Bhardwaj, Vaishali] Univ Washington, Dept Astron, Seattle, WA 98195 USA. [Burles, Scott] Cutler Grp LP, San Francisco, CA 94104 USA. [Chen, Yan-Mei; Tremonti, Christy A.] Univ Wisconsin, Dept Astron, Madison, WI 53706 USA. [Eisenstein, Daniel J.] Harvard Smithsonian Ctr Astrophys, Cambridge, MA 02138 USA. [Gunn, James E.; Knapp, G. R.; Loomis, Craig P.; Lupton, Robert H.; Strauss, Michael A.] Princeton Univ, Dept Astrophys Sci, Princeton, NJ 08544 USA. [Maraston, Claudia; Percival, Will J.; Thomas, Daniel] Univ Portsmouth, Inst Cosmol & Gravitat, Portsmouth PO1 3FX, Hants, England. [Muna, Demitri; Weaver, Benjamin A.] NYU, Ctr Cosmol & Particle Phys, New York, NY 10003 USA. [Myers, Adam D.] Univ Wyoming, Dept Phys & Astron, Laramie, WY 82071 USA. [Padmanabhan, Nikhil] Yale Univ, Dept Phys, New Haven, CT 06520 USA. [Paris, Isabelle; Petitjean, Patrick] UPMC, CNRS, Inst Astrophys Paris, UMR7095, F-75014 Paris, France. [Paris, Isabelle] Univ Chile, Dept Astron, Santiago, Chile. [Rockosi, Constance M.] Univ Calif Santa Cruz, UCO Lick Observ, Santa Cruz, CA 95064 USA. [Schneider, Donald P.] Penn State Univ, Dept Astron & Astrophys, University Pk, PA 16802 USA. [Schneider, Donald P.] Penn State Univ, Inst Gravitat, University Pk, PA 16802 USA. [Schneider, Donald P.] Penn State Univ, Cosmos, University Pk, PA 16802 USA. [Wake, David A.] Yale Univ, Dept Astron, New Haven, CT 06520 USA. [Wood-Vasey, W. Michael] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. RP Bolton, AS (reprint author), Univ Utah, Dept Phys & Astron, 115 South 1400 East, Salt Lake City, UT 84112 USA. EM bolton@astro.utah.edu FU PNPS; INSU FX This research has made use of the POLLUX database (http://pollux.graal.univ-montp2.fr) operated at LUPM (Universite Montpellier II - CNRS, France) with the support of the PNPS and INSU. NR 59 TC 228 Z9 229 U1 2 U2 10 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-6256 J9 ASTRON J JI Astron. J. PD NOV PY 2012 VL 144 IS 5 AR 144 DI 10.1088/0004-6256/144/5/144 PG 20 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 029XI UT WOS:000310530400020 ER PT J AU Gettings, DP Gonzalez, AH Stanford, SA Eisenhardt, PRM Brodwin, M Mancone, C Stern, D Zeimann, GR Masci, FJ Papovich, C Tanaka, I Wright, EL AF Gettings, Daniel P. Gonzalez, Anthony H. Stanford, S. Adam Eisenhardt, Peter R. M. Brodwin, Mark Mancone, Conor Stern, Daniel Zeimann, Gregory R. Masci, Frank J. Papovich, Casey Tanaka, Ichi Wright, Edward L. TI THE MASSIVE DISTANT CLUSTERS OF WISE SURVEY: THE FIRST DISTANT GALAXY CLUSTER DISCOVERED BY WISE SO ASTROPHYSICAL JOURNAL LETTERS LA English DT Article DE galaxies: clusters: individual (MOO J2342.0+1301); galaxies: distances and redshifts; galaxies: evolution ID STELLAR POPULATION SYNTHESIS; DIGITAL SKY SURVEY; DARK-MATTER; TELESCOPE; Z=1.75; RESOLUTION; EXISTENCE; UNIVERSE; CATALOG; MODELS AB We present spectroscopic confirmation of a z = 0.99 galaxy cluster discovered using data from the Wide-field Infrared Survey Explorer (WISE). This is the first z similar to 1 cluster candidate from the Massive Distant Clusters of WISE Survey to be confirmed. It was selected as an overdensity of probable z greater than or similar to 1 sources using a combination of WISE and Sloan Digital Sky Survey DR8 photometric catalogs. Deeper follow-up imaging data from Subaru and WIYN reveal the cluster to be a rich system of galaxies, and multi-object spectroscopic observations from Keck confirm five cluster members at z = 0.99. The detection and confirmation of this cluster represents a first step toward constructing a uniformly selected sample of distant, high-mass galaxy clusters over the full extragalactic sky using WISE data. C1 [Gettings, Daniel P.; Gonzalez, Anthony H.; Mancone, Conor] Univ Florida, Dept Astron, Bryant Space Ctr 211, Gainesville, FL 32611 USA. [Stanford, S. Adam] Lawrence Livermore Natl Lab, Inst Geophys & Planetary Phys, Livermore, CA 94550 USA. [Stanford, S. Adam; Zeimann, Gregory R.] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. [Eisenhardt, Peter R. M.; Stern, Daniel] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Brodwin, Mark] Univ Missouri, Dept Phys & Astron, Kansas City, MO 64110 USA. [Masci, Frank J.] CALTECH, Ctr Infrared Proc & Anal, Pasadena, CA 91125 USA. [Papovich, Casey] Texas A&M Univ, Dept Phys & Astron, College Stn, TX 77843 USA. [Papovich, Casey] Texas A&M Univ, George P & Cynthia Woods Mitchell Inst Fundamenta, College Stn, TX 77843 USA. [Tanaka, Ichi] Natl Inst Nat Sci, Natl Astron Observ Japan, Subaru Telescope, Hilo, HI 96720 USA. [Wright, Edward L.] UCLA Astron, Los Angeles, CA 90095 USA. RP Gettings, DP (reprint author), Univ Florida, Dept Astron, Bryant Space Ctr 211, Gainesville, FL 32611 USA. FU National Aeronautics and Space Administration (NASA); NASA Astrophysics Data Analysis Program (ADAP) [NNX12AE15G]; W.M. Keck Foundation FX The authors thank the anonymous referee whose comments improved the quality of the manuscript. This publication makes use of data products from the Wide-field Infrared Survey Explorer, which is a joint project of the University of California, Los Angeles and the Jet Propulsion Laboratory/California Institute of Technology, funded by the National Aeronautics and Space Administration (NASA). D. P. G. and A. H. G. acknowledge support for this research from the NASA Astrophysics Data Analysis Program (ADAP) through grant NNX12AE15G. Some of the data presented herein were obtained at the W. M. Keck Observatory, which is operated as a scientific partnership among the California Institute of Technology, the University of California and the National Aeronautics and Space Administration. The Observatory was made possible by the generous financial support of the W.M. Keck Foundation. Based in part on data collected at Subaru Telescope, which is operated by the National Astronomical Observatory of Japan. D. P. G. was a Visiting Astronomer, Kitt Peak National Observatory, National Optical Astronomy Observatory, which is operated by the Association of Universities for Research in Astronomy (AURA) under cooperative agreement with the National Science Foundation. The WIYN Observatory is a joint facility of the University of Wisconsin-Madison, Indiana University, Yale University, and the National Optical Astronomy Observatory. This research has made use of the NASA/IPAC Infrared Science Archive, which is operated by the Jet Propulsion Laboratory, California Institute of Technology, under contract with the National Aeronautics and Space Administration. NR 43 TC 11 Z9 11 U1 0 U2 4 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 2041-8205 EI 2041-8213 J9 ASTROPHYS J LETT JI Astrophys. J. Lett. PD NOV 1 PY 2012 VL 759 IS 1 AR L23 DI 10.1088/2041-8205/759/1/L23 PG 6 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 028XO UT WOS:000310458900023 ER PT J AU Rosa, BA Zhang, J Major, IT Qin, WS Chen, J AF Rosa, Bruce A. Zhang, Ji Major, Ian T. Qin, Wensheng Chen, Jin TI Optimal timepoint sampling in high-throughput gene expression experiments SO BIOINFORMATICS LA English DT Article ID WIDE TRANSCRIPTIONAL ANALYSIS; CELL-CYCLE; REGULATED GENES; BUDDING YEAST; TIME-SERIES; RNA-SEQ; JASMONATE; STRESS; REPRODUCIBILITY; INTERPOLATION AB Motivation: Determining the best sampling rates (which maximize information yield and minimize cost) for time-series high-throughput gene expression experiments is a challenging optimization problem. Although existing approaches provide insight into the design of optimal sampling rates, our ability to utilize existing differential gene expression data to discover optimal timepoints is compelling. Results: We present a new data-integrative model, Optimal Timepoint Selection (OTS), to address the sampling rate problem. Three experiments were run on two different datasets in order to test the performance of OTS, including iterative-online and a top-up sampling approaches. In all of the experiments, OTS outperformed the best existing timepoint selection approaches, suggesting that it can optimize the distribution of a limited number of timepoints, potentially leading to better biological insights about the resulting gene expression patterns. C1 [Rosa, Bruce A.; Qin, Wensheng] Lakehead Univ, Biorefining Res Inst, Thunder Bay, ON P7B 5E1, Canada. [Rosa, Bruce A.; Qin, Wensheng] Lakehead Univ, Dept Biol, Thunder Bay, ON P7B 5E1, Canada. [Rosa, Bruce A.; Major, Ian T.; Chen, Jin] Michigan State Univ, MSU DOE Plant Res Lab, E Lansing, MI 48824 USA. [Zhang, Ji] Univ So Queensland, Dept Math & Comp, Toowoomba, Qld 4350, Australia. [Chen, Jin] Michigan State Univ, Dept Comp Sci & Engn, E Lansing, MI 48824 USA. RP Qin, WS (reprint author), Lakehead Univ, Biorefining Res Inst, 955 Oliver Rd, Thunder Bay, ON P7B 5E1, Canada. EM wqin@lakeheadu.ca; jinchen@msu.edu FU U.S. Department of Energy (Chemical Sciences, Geosciences and Biosciences Division) [DE-FG02-91ER20021]; Natural Sciences and Engineering Research Council of Canada Research Development Fund, Canada FX This project has been funded by the U.S. Department of Energy (Chemical Sciences, Geosciences and Biosciences Division, grant no. DE-FG02-91ER20021 to J.C. and Natural Sciences and Engineering Research Council of Canada Research Development Fund, Canada to W.Q. NR 39 TC 2 Z9 2 U1 0 U2 8 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 1367-4803 J9 BIOINFORMATICS JI Bioinformatics PD NOV 1 PY 2012 VL 28 IS 21 BP 2773 EP 2781 DI 10.1093/bioinformatics/bts511 PG 9 WC Biochemical Research Methods; Biotechnology & Applied Microbiology; Computer Science, Interdisciplinary Applications; Mathematical & Computational Biology; Statistics & Probability SC Biochemistry & Molecular Biology; Biotechnology & Applied Microbiology; Computer Science; Mathematical & Computational Biology; Mathematics GA 025AR UT WOS:000310155300009 PM 22923305 ER PT J AU Hill, SM Lu, YL Molina, J Heiser, LM Spellman, PT Speed, TP Gray, JW Mills, GB Mukherjee, S AF Hill, Steven M. Lu, Yiling Molina, Jennifer Heiser, Laura M. Spellman, Paul T. Speed, Terence P. Gray, Joe W. Mills, Gordon B. Mukherjee, Sach TI Bayesian Inference of Signaling Network Topology in a Cancer Cell Line SO BIOINFORMATICS LA English DT Article ID GENE REGULATORY NETWORKS; VARIABLE SELECTION; EXPRESSION DATA; PRIOR KNOWLEDGE; PROTEIN ARRAY; PATHWAYS; MODELS; LASSO AB Motivation: Protein signaling networks play a key role in cellular function, and their dysregulation is central to many diseases, including cancer. To shed light on signaling network topology in specific contexts, such as cancer, requires interrogation of multiple proteins through time and statistical approaches to make inferences regarding network structure. Results: In this study, we use dynamic Bayesian networks to make inferences regarding network structure and thereby generate testable hypotheses. We incorporate existing biology using informative network priors, weighted objectively by an empirical Bayes approach, and exploit a connection between variable selection and network inference to enable exact calculation of posterior probabilities of interest. The approach is computationally efficient and essentially free of user-set tuning parameters. Results on data where the true, underlying network is known place the approach favorably relative to existing approaches. We apply these methods to reverse-phase protein array time-course data from a breast cancer cell line (MDA-MB-468) to predict signaling links that we independently validate using targeted inhibition. The methods proposed offer a general approach by which to elucidate molecular networks specific to biological context, including, but not limited to, human cancers. C1 [Lu, Yiling; Molina, Jennifer; Mills, Gordon B.] Univ Texas MD Anderson Canc Ctr, Dept Syst Biol, Houston, TX 77054 USA. [Hill, Steven M.; Mukherjee, Sach] Netherlands Canc Inst, Dept Biochem, NL-1066 CX Amsterdam, Netherlands. [Hill, Steven M.] Univ Warwick, Ctr Complex Sci, Coventry CV4 7AL, W Midlands, England. [Hill, Steven M.; Mukherjee, Sach] Univ Warwick, Dept Stat, Coventry CV4 7AL, W Midlands, England. [Heiser, Laura M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. [Spellman, Paul T.; Gray, Joe W.] Oregon Hlth & Sci Univ, Ctr Spatial Syst Biomed, Portland, OR 97239 USA. [Speed, Terence P.] Walter & Eliza Hall Inst Med Res, Bioinformat Div, Melbourne, Vic 3052, Australia. [Speed, Terence P.] Univ Calif Berkeley, Dept Stat, Berkeley, CA 94720 USA. RP Mills, GB (reprint author), Univ Texas MD Anderson Canc Ctr, Dept Syst Biol, Houston, TX 77054 USA. EM s.hill@nki.nl; gmills@mdanderson.org; s.mukherjee@nki.nl OI Hill, Steven/0000-0002-5909-692X FU U.S. Department of Energy [DE-AC02-05CH11231, NCI U54 CA 112970, NCI P50 CA 58207]; Stand Up to Cancer/AACR Dream Team Grant [SU2C-AACR- DT0209, NCI PO1CA099031, NCI P30 CA16672, KG 081694]; UK EPSRC [EP/E501311/1]; Cancer Systems Biology Center grant from the Netherlands Organisation for Scientific Research FX U.S. Department of Energy (Contract No. DE-AC02-05CH11231, NCI U54 CA 112970 and NCI P50 CA 58207 to J.W.G.); Stand Up to Cancer/AACR Dream Team Grant (SU2C-AACR- DT0209, NCI PO1CA099031, NCI P30 CA16672 and Komen Grant KG 081694 to G.B.M.); UK EPSRC EP/E501311/1 and the Cancer Systems Biology Center grant from the Netherlands Organisation for Scientific Research. The content is solely the responsibility of the authors and does not necessarily represent the official views of the NCI, NIH, AACR or Komen Foundation. NR 34 TC 35 Z9 36 U1 1 U2 20 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 1367-4803 J9 BIOINFORMATICS JI Bioinformatics PD NOV 1 PY 2012 VL 28 IS 21 BP 2804 EP 2810 DI 10.1093/bioinformatics/bts514 PG 7 WC Biochemical Research Methods; Biotechnology & Applied Microbiology; Computer Science, Interdisciplinary Applications; Mathematical & Computational Biology; Statistics & Probability SC Biochemistry & Molecular Biology; Biotechnology & Applied Microbiology; Computer Science; Mathematical & Computational Biology; Mathematics GA 025AR UT WOS:000310155300013 PM 22923301 ER PT J AU Dang, LX Annapureddy, HVR Sun, XQ Thallapally, PK McGrail, BP AF Dang, Liem X. Annapureddy, Harsha V. R. Sun, Xiuquan Thallapally, Praveen K. McGrail, B. Peter TI Understanding nanofluid stability through molecular simulation SO CHEMICAL PHYSICS LETTERS LA English DT Article ID METAL-ORGANIC FRAMEWORKS; WATER; ADSORPTION; DYNAMICS; DESIGN; GRAPHITE; LIQUIDS; STORAGE AB Molecular dynamics simulations were carried out to systematically study solvation and nanoparticle-particle interactions in n-hexane, water and methanol solvents. The dynamics of the n-hexane molecules was significantly influenced by the solvated nanoparticles. Water and methanol show significant structural signatures binding to the metal coordination sites of the nanoparticles while liquid hexane does not. The computed free energy profiles illustrate that the associations between nanoparticles in solution are stable and depend on the relative orientation of them. Also, these profiles indicate a low interaction potential between nanoparticles in methanol, confirming experimental observations of inherent nanofluid stability without need for added surfactant. Published by Elsevier B.V. C1 [Dang, Liem X.; Annapureddy, Harsha V. R.; Sun, Xiuquan; Thallapally, Praveen K.; McGrail, B. Peter] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Dang, LX (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM liem.dang@pnnl.gov RI Annapureddy, Harsha V R/E-9818-2013; thallapally, praveen/I-5026-2014 OI thallapally, praveen/0000-0001-7814-4467 FU US Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences; Office of Energy Efficiency and Renewable Energy, Geothermal Technologies Program FX This Letter was supported by the US Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences and by the Office of Energy Efficiency and Renewable Energy, Geothermal Technologies Program. Pacific Northwest National Laboratory (PNNL) is a multiprogram national laboratory operated for DOE by Battelle. NR 31 TC 6 Z9 6 U1 1 U2 39 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2614 EI 1873-4448 J9 CHEM PHYS LETT JI Chem. Phys. Lett. PD NOV 1 PY 2012 VL 551 BP 115 EP 120 DI 10.1016/j.cplett.2012.09.025 PG 6 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA 027OK UT WOS:000310362200023 ER PT J AU Williams, AP Funk, C Michaelsen, J Rauscher, SA Robertson, I Wils, THG Koprowski, M Eshetu, Z Loader, NJ AF Williams, A. Park Funk, Chris Michaelsen, Joel Rauscher, Sara A. Robertson, Iain Wils, Tommy H. G. Koprowski, Marcin Eshetu, Zewdu Loader, Neil J. TI Recent summer precipitation trends in the Greater Horn of Africa and the emerging role of Indian Ocean sea surface temperature SO CLIMATE DYNAMICS LA English DT Article DE African monsoon; Indian Ocean warming; Drought; Moisture transports; Energy flux; Tree rings; Stable isotopes; Global warming; Food security ID OXYGEN-ISOTOPE RATIOS; ATMOSPHERIC ENERGY TRANSPORTS; JUNE-SEPTEMBER RAINFALL; TREE-RING CELLULOSE; WEST-AFRICA; STABLE-ISOTOPES; GLOBAL PRECIPITATION; CLIMATE VARIABILITY; GAUGE OBSERVATIONS; ALPHA-CELLULOSE AB We utilize a variety of climate datasets to examine impacts of two mechanisms on precipitation in the Greater Horn of Africa (GHA) during northern-hemisphere summer. First, surface-pressure gradients draw moist air toward the GHA from the tropical Atlantic Ocean and Congo Basin. Variability of the strength of these gradients strongly influences GHA precipitation totals and accounts for important phenomena such as the 1960s-1980s rainfall decline and devastating 1984 drought. Following the 1980s, precipitation variability became increasingly influenced by the southern tropical Indian Ocean (STIO) region. Within this region, increases in sea-surface temperature, evaporation, and precipitation are linked with increased exports of dry mid-tropospheric air from the STIO region toward the GHA. Convergence of dry air above the GHA reduces local convection and precipitation. It also produces a clockwise circulation response near the ground that reduces moisture transports from the Congo Basin. Because precipitation originating in the Congo Basin has a unique isotopic signature, records of moisture transports from the Congo Basin may be preserved in the isotopic composition of annual tree rings in the Ethiopian Highlands. A negative trend in tree-ring oxygen-18 during the past half century suggests a decline in the proportion of precipitation originating from the Congo Basin. This trend may not be part of a natural cycle that will soon rebound because climate models characterize Indian Ocean warming as a principal signature of greenhouse-gas induced climate change. We therefore expect surface warming in the STIO region to continue to negatively impact GHA precipitation during northern-hemisphere summer. C1 [Williams, A. Park] Los Alamos Natl Lab, Div Earth & Environm Sci, Los Alamos, NM 87545 USA. [Williams, A. Park; Funk, Chris; Michaelsen, Joel] Univ Calif Santa Barbara, Dept Geog, Santa Barbara, CA 93106 USA. [Funk, Chris] US Geol Survey, Sioux Falls, SD USA. [Rauscher, Sara A.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Robertson, Iain; Loader, Neil J.] Swansea Univ, Coll Sci, Dept Geog, Swansea, W Glam, Wales. [Wils, Tommy H. G.] Rotterdam Univ, Dept Geog, Rotterdam, Netherlands. [Koprowski, Marcin] Nicholas Copernicus Univ, Lab Dendrochronol, Inst Ecol & Environm Protect, Torun, Poland. [Eshetu, Zewdu] Ethiopian Inst Agr Res, Forestry Res Ctr, Addis Ababa, Ethiopia. RP Williams, AP (reprint author), Los Alamos Natl Lab, Div Earth & Environm Sci, Los Alamos, NM 87545 USA. EM parkwilliams@lanl.gov RI Robertson, Iain/H-5327-2012; Koprowski, Marcin/A-2863-2014; Williams, Park/B-8214-2016 OI Robertson, Iain/0000-0001-7174-4523; Koprowski, Marcin/0000-0002-0583-4165; Williams, Park/0000-0001-8176-8166 FU U.S. Agency for International Development Famine Early Warning System Network under U.S. Geological Survey [G09AC00001]; National Aeronautics and Space Administration under Precipitation Science [NNX07AG266]; U.S. Department of Energy through the LANL/LDRD Program; Climate Change Consortium of Wales; Royal Society (UK); CHG FX This research was supported by the U.S. Agency for International Development Famine Early Warning System Network under U.S. Geological Survey Cooperative Agreement #G09AC00001 and the National Aeronautics and Space Administration under Precipitation Science Grant #NNX07AG266. Park Williams and Sara Rauscher gratefully acknowledge support from the U.S. Department of Energy through the LANL/LDRD Program. Iain Robertson is supported by the Climate Change Consortium of Wales. Marcin Koprowski was supported by an International Incoming Short Visit from the Royal Society (UK). Ethiopian precipitation data were provided by the Ethiopian Meteorological Agency. Thanks to Tufa Dinku for assisting the authors in obtaining this data purchase, providing the best possible foundation for an analysis of trends in Ethiopia. Thanks to Greg Husak for his invaluable part in obtaining CHG funding. Comments by Amy McNally, Brian Osborn, Charles Jones, Ellen Mosley-Thompson, Harikishan Jayanthi, Kevin Anchukaitis, Kyle Cavanaugh, Leila Carvalho, Lonnie Thompson, Naomi Levin, Tom Adamson, and two anonymous reviewers greatly improved the quality of the manuscript. NCEP/NCAR data were accessed online through the NOAA Earth System Research Laboratory (ESRL) Physical Sciences Division (PSD, http://www.esrl.noaa.gov/psd). ECMWF data were produced by the European Centre for Medium-Range Weather Forecasts ERA-40 project (http://www. data.ecmwf.int/data/). GHCN data were accessed from the National Climate Data Center (ftp://ncdc.noaa.gov/pub/data/ghcn/v2/). NR 91 TC 25 Z9 25 U1 4 U2 59 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0930-7575 J9 CLIM DYNAM JI Clim. Dyn. PD NOV PY 2012 VL 39 IS 9-10 BP 2307 EP 2328 DI 10.1007/s00382-011-1222-y PG 22 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 025VQ UT WOS:000310224400013 ER PT J AU Brandao, FGSL Christandl, M Yard, J AF Brandao, Fernando G. S. L. Christandl, Matthias Yard, Jon TI Faithful Squashed Entanglement (vol 306, pg 805, 2011) SO COMMUNICATIONS IN MATHEMATICAL PHYSICS LA English DT Correction C1 [Brandao, Fernando G. S. L.] Univ Fed Minas Gerais, Dept Fis, BR-30123970 Belo Horizonte, MG, Brazil. [Christandl, Matthias] Swiss Fed Inst Technol, Inst Theoret Phys, CH-8057 Zurich, Switzerland. [Yard, Jon] Los Alamos Natl Lab, Ctr Nonlinear Studies CNLS, Los Alamos, NM 87545 USA. RP Brandao, FGSL (reprint author), Univ Fed Minas Gerais, Dept Fis, Caixa Postal 702, BR-30123970 Belo Horizonte, MG, Brazil. EM fgslbrandao@gmail.com; christandl@phys.ethz.ch; jtyard@lanl.gov RI Christandl, Matthias/L-8830-2014 OI Christandl, Matthias/0000-0003-2281-3355 NR 1 TC 4 Z9 4 U1 0 U2 2 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0010-3616 J9 COMMUN MATH PHYS JI Commun. Math. Phys. PD NOV PY 2012 VL 316 IS 1 BP 287 EP 288 DI 10.1007/s00220-012-1584-y PG 2 WC Physics, Mathematical SC Physics GA 027HD UT WOS:000310342200011 ER PT J AU Planes, A Lloveras, P Castan, T Saxena, A Porta, M AF Planes, Antoni Lloveras, Pol Castan, Teresa Saxena, Avadh Porta, Marcel TI Ginzburg-Landau modelling of precursor nanoscale textures in ferroelastic materials SO CONTINUUM MECHANICS AND THERMODYNAMICS LA English DT Article DE Ferroelastic; Martensite; Precursors; Tweed; Strain glass ID SHAPE-MEMORY ALLOYS; MARTENSITIC TRANSFORMATIONS; TRANSITIONS; DISORDER; POINT AB A Ginzburg-Landau free-energy model is proposed to study spatially inhomogeneous states that often occur as precursors of ferroelastic/martensitic transitions. Disorder is included in the harmonic coefficient of the free-energy density which gives rise to a spatial distribution of transition temperatures, and lattice integrity is imposed through Saint-V,nant compatibility conditions which lead to a long-range anisotropic elastic interaction. We show that precursor textures are a result of the competition between elastic anisotropy and disorder. Cross-hatched modulations (tweed patterns) take place for temperatures above the martensitic phase in the limit of high anisotropy and/or low disorder while a nano-cluster phase-separated state occurs at low anisotropies or high disorder. In the latter case, nanoscale inhomogeneities give rise to glassy behaviour while the structural transition is inhibited. Interestingly, in this case, the ferroelastic system also displays a large thermo-mechanical response so that the low-symmetry structure can be easily induced by the application of relatively small stresses within a broad temperature range. C1 [Planes, Antoni; Lloveras, Pol; Castan, Teresa] Univ Barcelona, Dept Estruct & Constituents Mat, Fac Fis, E-08028 Barcelona, Catalonia, Spain. [Saxena, Avadh; Porta, Marcel] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Planes, A (reprint author), Univ Barcelona, Dept Estruct & Constituents Mat, Fac Fis, Diagonal 647, E-08028 Barcelona, Catalonia, Spain. EM toni@ecm.ub.es RI Lloveras, Pol/M-3775-2014; Planes, Antoni/O-1904-2015; OI Lloveras, Pol/0000-0003-4133-2223; Planes, Antoni/0000-0001-5213-5714; Porta Tena, Marcel/0000-0001-7582-9671 FU Spanish Ministery of Innovation and Science [MAT2010-15114]; U.S. Department of Energy FX This work has received financial support from Spanish Ministery of Innovation and Science, project MAT2010-15114 and the U.S. Department of Energy. NR 29 TC 3 Z9 3 U1 0 U2 21 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0935-1175 J9 CONTINUUM MECH THERM JI Continuum Mech. Thermodyn. PD NOV PY 2012 VL 24 IS 4-6 SI SI BP 619 EP 627 DI 10.1007/s00161-011-0203-z PG 9 WC Thermodynamics; Mechanics SC Thermodynamics; Mechanics GA 027AY UT WOS:000310325400023 ER PT J AU Otter, RR Bailey, FC Fortner, AM Adams, SM AF Otter, Ryan R. Bailey, Frank C. Fortner, Allison M. Adams, S. Marshall TI Trophic status and metal bioaccumulation differences in multiple fish species exposed to coal ash-associated metals SO ECOTOXICOLOGY AND ENVIRONMENTAL SAFETY LA English DT Article DE Coal ash; Arsenic; Selenium; Bioaccumulation; Food web; Trophic dynamics ID SAN-FRANCISCO BAY; FLY-ASH; SELENIUM BIOACCUMULATION; AQUATIC ECOSYSTEMS; CLARIAS-BATRACHUS; STABLE-ISOTOPES; POWER-PLANT; FOOD WEBS; TOXICITY; SUNFISH AB On December 22, 2008 a dike containing coal fly ash from the Tennessee Valley Authority Kingston Fossil Plant near Kingston Tennessee USA failed and resulted in the largest coal ash spill in U.S. history. Coal ash, a by-product of coal combustion, is known to contain multiple contaminants of concern, including arsenic and selenium. The purpose of this study was to investigate species differences in the bioaccumulation of arsenic and selenium and potential factors contributing to these differences (i.e., trophic dynamics and gut pH) in the vicinity of the Kingston coal ash spill. Elevated levels of arsenic and selenium were observed in various tissues of largemouth bass, white crappie, bluegill and redear sunfish from sites associated with the Kingston coal ash spill. Highest concentrations of selenium were found in redear sunfish with liver concentrations as high as 24.83 mg/kg dry weight and ovary concentrations up to 10.40 mg/kg dry weight at coal ash-associated sites. Investigations into the gut pH and trophic dynamics of redear sunfish and bluegill demonstrated a large difference in the gut physiology between these two species. Redear sunfish stomach and intestinal pH was found to be 1.1 and 0.16 pH units higher than in bluegill, respectively. In addition, fish from coal ash-associated sites showed enrichment differences (N-15 and C-13) compared to no ash sites, indicating differences in food web dynamics between sites. These results imply the incorporation of coal ash-associated compounds into local food webs and/or a shift in diet at ash sites compared to the no ash reference sites. Based on these results, further investigation into a broader food web at ash-associated sites is warranted. (C) 2012 Elsevier Inc. All rights reserved. C1 [Otter, Ryan R.; Bailey, Frank C.] Middle Tennessee State Univ, Dept Biol, Murfreesboro, TN 37132 USA. [Fortner, Allison M.] ARCADIS US Inc, Knoxville, TN 37934 USA. [Adams, S. Marshall] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. RP Otter, RR (reprint author), Middle Tennessee State Univ, Dept Biol, 1500 Greenland Dr, Murfreesboro, TN 37132 USA. EM Ryan.Otter@mtsu.edu; Frank.Bailey@mtsu.edu; fortneram@ornl.gov; marshalladams3@comcast.net FU Tennessee Valley Authority at the Kingston Tennessee fossil fuel plant; UT-Battelle for the US DOE [DE-ACO5-000R22725] FX This study was funded by the Tennessee Valley Authority as part of a larger project investigating the environmental consequences of the coal ash spill at the Kingston Tennessee fossil fuel plant. The Oak Ridge National Laboratory is managed by UT-Battelle for the US DOE under contract number DE-ACO5-000R22725. NR 50 TC 13 Z9 14 U1 3 U2 43 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0147-6513 J9 ECOTOX ENVIRON SAFE JI Ecotox. Environ. Safe. PD NOV 1 PY 2012 VL 85 BP 30 EP 36 DI 10.1016/j.ecoenv.2012.08.022 PG 7 WC Environmental Sciences; Toxicology SC Environmental Sciences & Ecology; Toxicology GA 025JY UT WOS:000310186300004 PM 22947506 ER PT J AU Cao, B Majors, PD Ahmed, B Renslow, RS Silvia, CP Shi, L Kjelleberg, S Fredrickson, JK Beyenal, H AF Cao, Bin Majors, Paul D. Ahmed, Bulbul Renslow, Ryan S. Silvia, Crystal P. Shi, Liang Kjelleberg, Staffan Fredrickson, Jim K. Beyenal, Haluk TI Biofilm shows spatially stratified metabolic responses to contaminant exposure SO ENVIRONMENTAL MICROBIOLOGY LA English DT Article ID SHEWANELLA-ONEIDENSIS MR-1; EXTRACELLULAR POLYMERIC SUBSTANCES; PSEUDOMONAS-AERUGINOSA BIOFILMS; NUCLEAR-MAGNETIC-RESONANCE; SP HRCR-1 BIOFILMS; MICROBIAL BIOFILMS; REDUCTION; IMMOBILIZATION; NMR; MICROELECTRODES AB Biofilms are core to a range of biological processes, including the bioremediation of environmental contaminants. Within a biofilm population, cells with diverse genotypes and phenotypes coexist, suggesting that distinct metabolic pathways may be expressed based on the local environmental conditions in a biofilm. However, metabolic responses to local environmental conditions in a metabolically active biofilm interacting with environmental contaminants have never been quantitatively elucidated. In this study, we monitored the spatiotemporal metabolic responses of metabolically active Shewanella oneidensis MR-1 biofilms to U(VI) (uranyl, UO22+) and Cr(VI) (chromate, CrO42-) using non-invasive nuclear magnetic resonance imaging (MRI) and spectroscopy (MRS) approaches to obtain insights into adaptation in biofilms during biofilm-contaminant interactions. While overall biomass distribution was not significantly altered upon exposure to U(VI) or Cr(VI), MRI and spatial mapping of the diffusion revealed localized changes in the water diffusion coefficients in the biofilms, suggesting significant contaminant-induced changes in structural or hydrodynamic properties during bioremediation. Finally, we quantitatively demonstrated that the metabolic responses of biofilms to contaminant exposure are spatially stratified, implying that adaptation in biofilms is custom-developed based on local microenvironments. C1 [Cao, Bin; Ahmed, Bulbul; Renslow, Ryan S.; Beyenal, Haluk] Washington State Univ, Gene & Linda Voiland Sch Chem Engn & Bioengn, Pullman, WA 99164 USA. [Cao, Bin; Majors, Paul D.; Silvia, Crystal P.; Shi, Liang; Fredrickson, Jim K.] Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99352 USA. [Cao, Bin; Kjelleberg, Staffan] Nanyang Technol Univ, SCELSE, Singapore, Singapore. [Cao, Bin] Nanyang Technol Univ, Sch Civil & Environm Engn, Singapore, Singapore. [Silvia, Crystal P.] Univ Washington, Seattle, WA 98195 USA. RP Beyenal, H (reprint author), Washington State Univ, Gene & Linda Voiland Sch Chem Engn & Bioengn, Pullman, WA 99164 USA. EM beyenal@wsu.edu RI Cao, Bin/H-2639-2012; Renslow, Ryan/E-5851-2010; Kjelleberg, Staffan/C-9229-2015 OI Cao, Bin/0000-0002-9462-496X; Renslow, Ryan/0000-0002-3969-5570; Kjelleberg, Staffan/0000-0003-4271-6413 FU US DOE Office of Biological and Environmental Research under the Subsurface Biogeochemistry Research (SBR) Program [DE-FG92-08ER64560]; DOE-BER SBR Program's Scientific Focus Area (SFA) at the Pacific Northwest National Laboratory (PNNL); NIEHS/NIH [21R01ES017070-01]; DOE's Office of Biological and Environmental Research; DOE [DE-AC05-76RL01830] FX The research was supported by the US DOE Office of Biological and Environmental Research under the Subsurface Biogeochemistry Research (SBR) Program (Grant DE-FG92-08ER64560), the DOE-BER SBR Program's Scientific Focus Area (SFA) at the Pacific Northwest National Laboratory (PNNL), and NIEHS/NIH (Grant 21R01ES017070-01). A portion of the research was performed in the William R. Wiley Environmental Molecular Sciences Laboratory, a national scientific user facility sponsored by the DOE's Office of Biological and Environmental Research and located at PNNL. PNNL is operated by Battelle for the DOE under Contract DE-AC05-76RL01830. NR 46 TC 24 Z9 24 U1 2 U2 64 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1462-2912 J9 ENVIRON MICROBIOL JI Environ. Microbiol. PD NOV PY 2012 VL 14 IS 11 BP 2901 EP 2910 DI 10.1111/j.1462-2920.2012.02850.x PG 10 WC Microbiology SC Microbiology GA 029DR UT WOS:000310475500004 PM 22925136 ER PT J AU Schmid, TE Eskenazi, B Marchetti, F Young, S Weldon, RH Baumgartner, A Anderson, D Wyrobek, AJ AF Schmid, Thomas E. Eskenazi, Brenda Marchetti, Francesco Young, Suzanne Weldon, Rosana H. Baumgartner, Adolf Anderson, Diana Wyrobek, Andrew J. TI Micronutrients intake is associated with improved sperm DNA quality in older men SO FERTILITY AND STERILITY LA English DT Article DE Human sperm alkaline and neutral Comet assay; vitamin C; vitamin E; beta-carotene; zinc; folate ID HEALTHY NONSMOKING MEN; OXIDATIVE STRESS; COMET ASSAY; MALE AGE; ANTIOXIDANT INTAKE; HUMAN-LYMPHOCYTES; SEMEN QUALITY; CHROMATIN INTEGRITY; HUMAN SPERMATOZOA; FOOD MUTAGENS AB Objective: To investigate whether lifestyle factors such as increased dietary intake of micronutrients reduce the risks of sperm DNA damage, and whether older men benefit more than younger men. Design: Cross-sectional study design with equalized assignments into age groups. Setting: National laboratory and university. Patient(s): Nonclinical group of 22-80-year-old nonsmoking men (n = 80) who reported no fertility problems. Main Outcome Measure(s): Sperm DNA damage measured by alkaline and neutral DNA electrophoresis (i.e., sperm Comet assay). Result(s): Sociodemographics, occupational exposures, medical and reproductive histories, and lifestyle habits were determined by questionnaire. The average daily dietary and supplement intake of micronutrients (vitamin C, vitamin E, b-carotene, zinc, and folate) was determined using the 100-item Modified Block Food Frequency Questionnaire (FFQ). Men with the highest intake of vitamin C had approximately 16% less sperm DNA damage (alkaline sperm Comet) than men with the lowest intake, with similar findings for vitamin E, folate, and zinc (but not beta-carotene). Older men (>44 years) with the highest vitamin C intake had approximately 20% less sperm DNA damage compared with older men with the lowest intake, with similar findings for vitamin E and zinc. The older men with the highest intake of these micronutrients showed levels of sperm damage that were similar to those of the younger men. However, younger men (<44 years) did not benefit from higher intakes of the micronutrients surveyed. Conclusion(s): Men with higher dietary and supplement intake of certain micronutrients may produce sperm with less DNA damage, especially among older men. This raises the broader question of how lifestyle factors, including higher intakes of antioxidants and micronutrients, might protect somatic as well as germ cells against age-associated genomic damage. (Fertil Steril (R) 2012;98:1130-7. (C) 2012 by American Society for Reproductive Medicine.) C1 [Schmid, Thomas E.; Marchetti, Francesco; Wyrobek, Andrew J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. [Schmid, Thomas E.; Marchetti, Francesco; Wyrobek, Andrew J.] Lawrence Livermore Natl Lab, Biosci Directorate, Livermore, CA USA. [Eskenazi, Brenda; Young, Suzanne; Weldon, Rosana H.] Univ Calif Berkeley, Sch Publ Hlth, Ctr Environm Res & Childrens Hlth, Berkeley, CA 94720 USA. [Baumgartner, Adolf; Anderson, Diana] Univ Bradford, Div Med Sci, Bradford BD7 1DP, W Yorkshire, England. RP Wyrobek, AJ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, 1 Cyclotron Rd,Mail Stop 977, Berkeley, CA 94720 USA. EM ajwyrobek@lbl.gov RI Anderson, Diana/J-6472-2015; OI Anderson, Diana/0000-0001-9673-0398; Marchetti, Francesco/0000-0002-9435-4867 FU National Institute of Environmental Health Sciences Superfund [P42ES04705]; US Department of Energy by Lawrence Livermore National Laboratory [W-7405-ENG-48]; Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; European Community [QLG4-CT-2002-51611] FX This work was performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under contract no. W-7405-ENG-48, with funding from National Institute of Environmental Health Sciences Superfund P42ES04705. This work was also performed at the Lawrence Berkeley National Laboratory under contract no. DE-AC02-05CH11231. A.B. was a Marie Curie fellow, European Community contract no. QLG4-CT-2002-51611. NR 53 TC 19 Z9 20 U1 2 U2 16 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 0015-0282 J9 FERTIL STERIL JI Fertil. Steril. PD NOV PY 2012 VL 98 IS 5 BP 1130 EP + DI 10.1016/j.fertnstert.2012.07.1126 PG 9 WC Obstetrics & Gynecology; Reproductive Biology SC Obstetrics & Gynecology; Reproductive Biology GA 028TW UT WOS:000310447300018 PM 22935557 ER PT J AU Person, M Hofstra, A Sweetkind, D Stone, W Cohen, D Gable, CW Banerjee, A AF Person, M. Hofstra, A. Sweetkind, D. Stone, W. Cohen, D. Gable, C. W. Banerjee, A. TI Analytical and numerical models of hydrothermal fluid flow at fault intersections SO GEOFLUIDS LA English DT Article DE convection; faults; groundwater; numerical modeling ID EXTENSIONAL GEOTHERMAL SYSTEMS; GROUNDWATER-FLOW; GREAT-BASIN; THERMAL-CONVECTION; NEVADA; MINERALIZATION; PERMEABILITY; BEOWAWE; CIRCULATION; TRANSPORT AB Fault intersections are the locus of hot spring activity and Carlin-type gold mineralization within the Basin and Range, USA. Analytical and numerical solutions to Stokes equation suggest that peak fluid velocities at fault intersections increase between 20% and 47% when fracture apertures have identical widths but increase by only about 1% and 8% when aperture widths vary by a factor of 2. This suggests that fault zone intersections must have enlarged apertures. Three-dimensional finite element models that consider intersecting 10- to 20-m wide fault planes resulted in hot spring activity being preferentially located at fault zone intersections when fault zones were assigned identical permeabilities. We found that the onset of convection at the intersections of the fault zones occurred in our hydrothermal model over a narrow permeability range between 5 x 10-13 and 7 x 10-13 m2. Relatively high vertical fluid velocities (0.33 m year-1) extended away from the fault intersections for about 0.51.5 km. For the boundary conditions and fault plane dimensions used, peak discharge temperatures of 112 degrees C at the water table occurred with an intermediate fault zone permeability of 5 x 10-13 m2. When fault plane permeability differed by a factor of 2 or more, the locus of hot spring activity shifted away from the intersections. However, increasing the permeability at the core of the fault plane intersection by 40% shifted the discharge back to the intersections. When aquifer units were assigned a permeability value equal to those of the fault planes, convective rolls developed that extend about 3 km laterally along the fault plane and into the adjacent aquifer. C1 [Person, M.; Banerjee, A.] New Mexico Inst Min & Technol, Dept Earth & Environm Sci, Socorro, NM 87801 USA. [Hofstra, A.; Sweetkind, D.] US Geol Survey, Denver, CO 80225 USA. [Stone, W.] New Mexico Inst Min & Technol, Dept Math, Socorro, NM 87801 USA. [Cohen, D.] Univ Geneva, Inst Environm Sci, Carouge, Switzerland. [Gable, C. W.] Los Alamos Natl Lab, Computat Earth Sci Grp, Los Alamos, NM USA. RP Person, M (reprint author), New Mexico Inst Min & Technol, Dept Earth & Environm Sci, Socorro, NM 87801 USA. EM mperson@nmt.edu RI Banerjee, Amlan/P-9658-2016; OI Banerjee, Amlan/0000-0002-2065-1391; Sweetkind, Donald/0000-0003-0892-4796; Gable, Carl/0000-0001-7063-0815 FU Department of Energy IGPP program; National Science Foundation [NSF-EAR 0809644]; U.S. Geological Survey Minerals Program FX We thank Mark Coolbaugh for his insights into Basin and Range geothermal systems and for the insightful review of Dr. Andy Manning of the USGS as well as two anonymous reviewers. This research was supported by the Department of Energy IGPP program under a grant to Carl Gable and Mark Person, the National Science Foundation under grant NSF-EAR 0809644 to Mark Person and Albert Hofstra, and by the U.S. Geological Survey Minerals Program, which funded the Metallogeny of the Great Basin project. NR 63 TC 10 Z9 10 U1 1 U2 31 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1468-8115 J9 GEOFLUIDS JI Geofluids PD NOV PY 2012 VL 12 IS 4 DI 10.1111/gfl.12002 PG 16 WC Geochemistry & Geophysics; Geology SC Geochemistry & Geophysics; Geology GA 029DC UT WOS:000310474000004 ER PT J AU Scullin, CS Partridge, LD AF Scullin, Chessa S. Partridge, L. Donald TI Modulation by pregnenolone sulfate of filtering properties in the hippocampal trisynaptic circuit SO HIPPOCAMPUS LA English DT Article DE gamma; theta; bandpass filter; lowpass filter; neurosteroid ID NEUROSTEROID-INDUCED ENHANCEMENT; SCHAFFER COLLATERAL SYNAPSES; SHORT-TERM FACILITATION; NATURAL SPIKE TRAINS; GAMMA-OSCILLATIONS; PYRAMIDAL CELLS; ENTORHINAL CORTEX; ACETYLCHOLINE-RECEPTORS; PRESYNAPTIC TERMINALS; INHIBITORY CIRCUITS AB Short-term synaptic plasticity alters synaptic efficacy on a timescale that is relevant to encoding information in spike trains. The dynamics of this plasticity, combined with that of the feedback and feedforward contributions of local interneurons, impose frequency-dependent properties on neuronal networks with implications for nervous system function. The trisynaptic network of the hippocampus is especially well suited to selectively filter components of frequency-dependent signals that are transmitted from the entorhinal cortex. We measured presynaptic [Ca2+]i in perforant path, mossy fiber, or Schaffer collateral terminals while simultaneously measuring field potentials of principal cells of the dentate, CA3, or CA1 synaptic fields over a range of stimulus frequencies of 2 to 77 Hz. In all three synaptic fields, the average [Ca2+]i during a 500 ms stimulus train rose monotonically with stimulus frequency. The average population spike amplitude during this stimulus train, however, exhibited a non-linear relationship to frequency that was distinct for each of the three synaptic fields. The dentate synaptic field exhibited the characteristics of a low pass filter, while both CA synaptic fields had bandpass filter characteristics with a gain that was greater than 1 in the passband frequencies. Importantly, alteration of the dynamic properties of this network could significantly impact information processing performed by the hippocampus. Pregnenolone sulfate (PregS), has frequency-dependent effects on paired- and multipulse plasticity in the dentate and CA1 synaptic fields of the hippocampal formation. We investigated the PregS-dependent modulation of the dynamic properties of transmission by the principal cells of the three hippocampal synaptic fields. Importantly, PregS is capable of altering the pattern separation capabilities that may underlie hippocampal information processing. (c) 2012 Wiley Periodicals, Inc. C1 [Partridge, L. Donald] Univ New Mexico, Sch Med, Dept Neurosci, Albuquerque, NM 87131 USA. [Scullin, Chessa S.] Lawrence Berkeley Natl Lab, Joint BioEnergy Inst, Phys Biosci Div, Emeryville, CA USA. [Scullin, Chessa S.] Sandia Natl Labs, Biomass Sci & Convers Technol Dept, Livermore, CA USA. RP Partridge, LD (reprint author), Univ New Mexico, Sch Med, Dept Neurosci, Albuquerque, NM 87131 USA. EM dpartridge@salud.unm.edu FU National Institutes of Health [MH07387] FX Grant sponsor: National Institutes of Health; Grant number: MH07387 NR 55 TC 3 Z9 6 U1 0 U2 5 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1050-9631 J9 HIPPOCAMPUS JI Hippocampus PD NOV PY 2012 VL 22 IS 11 BP 2184 EP 2198 DI 10.1002/hipo.22038 PG 15 WC Neurosciences SC Neurosciences & Neurology GA 026ZB UT WOS:000310320500009 PM 22648992 ER PT J AU Wasden, DL Moradi, H Farhang-Boroujeny, B AF Wasden, Daryl Leon Moradi, Hussein Farhang-Boroujeny, Behrouz TI Design and Implementation of an Underlay Control Channel for Cognitive Radios SO IEEE JOURNAL ON SELECTED AREAS IN COMMUNICATIONS LA English DT Article DE Cognitive Radio; Control Channel; Spread Spectrum Communication; Filter Banks ID AD HOC NETWORKS; WIRELESS NETWORKS; MULTICARRIER; COMMUNICATION; PERFORMANCE; SYSTEM; CDMA; OFDM; MAC AB Implementation of any cognitive radio network requires an effective control channel that can operate under various modes of activity from the primary users. This paper reports the design and implementation of a filter bank multicarrier spread spectrum (FBMC-SS) system for use as the control channel in cognitive radio networks. The proposed design is based on a filtered multitone (FMT) implementation. Carrier and timing acquisition and tracking methods as well as a blind channel estimation method are developed for the proposed control channel. We also report an implementation of the proposed FBMC-SS system on a hardware platform; a FlexRIO FPGA module from National Instruments. C1 [Wasden, Daryl Leon; Farhang-Boroujeny, Behrouz] Univ Utah, Elect & Comp Engn Dept, Salt Lake City, UT 84112 USA. [Moradi, Hussein] Idaho Natl Lab, Idaho Falls, ID 83415 USA. RP Wasden, DL (reprint author), Univ Utah, Elect & Comp Engn Dept, Salt Lake City, UT 84112 USA. EM wasden@ece.utah.edu; hussein.moradi@inl.gov; farhang@ece.utah.edu FU National Science Foundation [0750758]; U.S. Department of Energy [DE-AC07-05ID14517] FX This material is partially based upon work supported by the National Science Foundation Graduate Research Fellowship under Grant No. 0750758. This manuscript has been authored by Battelle Energy Alliance, LLC under Contract No. DE-AC07-05ID14517 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. NR 41 TC 14 Z9 14 U1 1 U2 6 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0733-8716 J9 IEEE J SEL AREA COMM JI IEEE J. Sel. Areas Commun. PD NOV PY 2012 VL 30 IS 10 BP 1875 EP 1889 DI 10.1109/JSAC.2012.121104 PG 15 WC Engineering, Electrical & Electronic; Telecommunications SC Engineering; Telecommunications GA 027DP UT WOS:000310332300004 ER PT J AU Allee, G Tschudi, W AF Allee, Guy Tschudi, William TI Edison Redux SO IEEE POWER & ENERGY MAGAZINE LA English DT Article DE DC technologies; History; Power demand; Power distribution; Power grids C1 [Allee, Guy] Intel Labs, Rio Rancho, NM USA. [Tschudi, William] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Allee, G (reprint author), Intel Labs, Rio Rancho, NM USA. NR 6 TC 38 Z9 40 U1 0 U2 5 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 1540-7977 J9 IEEE POWER ENERGY M JI IEEE Power Energy Mag. PD NOV-DEC PY 2012 VL 10 IS 6 BP 50 EP 59 DI 10.1109/MPE.2012.2212607 PG 10 WC Engineering, Electrical & Electronic SC Engineering GA 027HJ UT WOS:000310342800007 ER PT J AU Tang, LX Che, P Wang, JH AF Tang, Lixin Che, Ping Wang, Jianhui TI Corrective Unit Commitment to an Unforeseen Unit Breakdown SO IEEE TRANSACTIONS ON POWER SYSTEMS LA English DT Article DE Bundle methods; corrective scheduling; Lagrangian relaxation; scenarios; stochastic unit commitment; unforeseen breakdown ID STOCHASTIC-PROGRAMMING APPROACH; LAGRANGEAN DECOMPOSITION; DISRUPTION MANAGEMENT; OPTIMIZATION; RELAXATION; CONSTRAINTS; RECOVERY; BOUNDS; MODEL AB We investigate the corrective unit commitment problem to deal with disruption in power system operations caused by an unforeseen unit breakdown with stochastic duration. Since the original unit schedule is no longer feasible when a unit breaks down during operation, a corrective scheduling that provides an immediate response to such a disruption is needed to update the original schedule in time. The objective of the corrective scheduling is to minimize the generation cost and the deviation from the original schedule. The corrective scheduling problem is formulated as a mixed integer nonlinear programming model where the stochastic duration is expressed by tree-structured duration scenarios. The proposed variable splitting-based Lagrangian relaxation algorithm decomposes the problem into multiple single-unit subproblems and a linear programming-type artificial variable subproblem. Each single-unit subproblem is solved by a two-stage procedure. In the first stage, the generating level of the unit in each committed period is determined optimally. In the second stage, before the dynamic programming is called, an effective pre-processing technique based on optimality conditions is applied to speed up the procedure. The dual problem is solved by a bundle method. The numerical results show that the algorithm can find solutions very close to optimums within a reasonable time. C1 [Tang, Lixin; Che, Ping] Northeastern Univ, Logist Inst, Liaoning Key Lab Mfg Syst & Logist, Dept Math, Shenyang 110004, Peoples R China. [Wang, Jianhui] Argonne Natl Lab, Decis & Informat Sci Div, Argonne, IL 60439 USA. RP Tang, LX (reprint author), Northeastern Univ, Logist Inst, Liaoning Key Lab Mfg Syst & Logist, Dept Math, Shenyang 110004, Peoples R China. EM qhjytlx@mail.neu.edu.cn; cheping@mail.neu.edu.cn; jianhui.wang@anl.gov FU National Natural Science Foundation of China [71032004] FX This work was supported in part by the State Key Program of National Natural Science Foundation of China (71032004). Paper no. TPWRS-00502-2010. NR 28 TC 5 Z9 5 U1 2 U2 16 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0885-8950 J9 IEEE T POWER SYST JI IEEE Trans. Power Syst. PD NOV PY 2012 VL 27 IS 4 BP 1729 EP 1740 DI 10.1109/TPWRS.2011.2167523 PG 12 WC Engineering, Electrical & Electronic SC Engineering GA 027YC UT WOS:000310389000002 ER PT J AU Liu, C Wang, JH Ostrowski, J AF Liu, Cong Wang, Jianhui Ostrowski, James TI Static Switching Security in Multi-Period Transmission Switching SO IEEE TRANSACTIONS ON POWER SYSTEMS LA English DT Article DE Disjunctive programming; mixed-integer linear programming; static security analysis; transmission switching ID CONSTRAINED UNIT COMMITMENT; OPTIMAL POWER-FLOW; MARKET AB Transmission switching can improve the economic benefits of a power system through changing its topology during operations. However, the switching operation itself represents a step change in power systems, which is, to some extent, similar to a contingency that can bring disturbances into systems. This paper proposes a new model for multi-period, static-security-constrained transmission switching. Because the power flow on the network will be redistributed instantaneously after the switching operations, the new model involves using disjunctive programming, which considers two sets of power flow equations under possibly different topologies before/after switching. Each switchable transmission element is modeled into four actions or disjunctions. An action transition diagram coupling of four actions in different hours is used to represent feasible paths of instantaneous changes in the element status. Disjunctive formulations are transformed into mixed-integer programming problems. We compare the difference of the previous transmission switching model and the proposed one by using several numerical tests and verify the effectiveness of our solution methodology in the six-bus and RTS-96 systems. C1 [Liu, Cong; Wang, Jianhui; Ostrowski, James] Argonne Natl Lab, Decis & Informat Sci Div, Argonne, IL 60439 USA. [Liu, Cong; Wang, Jianhui; Ostrowski, James] Univ Tennessee, Knoxville, TN 37996 USA. RP Liu, C (reprint author), Argonne Natl Lab, Decis & Informat Sci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM liuc@anl.gov; jianhui.wang@anl.gov; jostrows@utk.edu OI Ostrowski, James/0000-0001-5636-555X FU U.S. Department of Energy, Office of Electricity Delivery and Energy FX This work is supported by the U.S. Department of Energy, Office of Electricity Delivery and Energy. Paper no. TPWRS-00535-2011. NR 26 TC 13 Z9 13 U1 1 U2 15 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0885-8950 J9 IEEE T POWER SYST JI IEEE Trans. Power Syst. PD NOV PY 2012 VL 27 IS 4 BP 1850 EP 1858 DI 10.1109/TPWRS.2012.2192486 PG 9 WC Engineering, Electrical & Electronic SC Engineering GA 027YC UT WOS:000310389000014 ER PT J AU Troy, N Flynn, D Milligan, M O'Malley, M AF Troy, Niamh Flynn, Damian Milligan, Michael O'Malley, Mark TI Unit Commitment With Dynamic Cycling Costs SO IEEE TRANSACTIONS ON POWER SYSTEMS LA English DT Article DE Power system modeling; thermal power generation ID THERMAL UNIT; DISPATCH AB Increased competition in the electricity sector and the integration of variable renewable energy sources is resulting in more frequent cycling of thermal plant. Thus, the wear-and-tear to generator components and the related costs are a growing concern for plant owners and system operators alike. This paper presents a formulation that can be implemented in a MIP dispatch model to dynamically model cycling costs based on unit operation. When implemented for a test system, the results show that dynamically modeling cycling costs reduces cycling operation and tends to change the merit order over time. This leads to the burden of cycling operation being more evenly distributed over the plant portfolio and reduces the total system costs relative to the case when cycling costs are not modeled. C1 [Troy, Niamh; Flynn, Damian; O'Malley, Mark] Univ Coll Dublin, Sch Elect Elect & Commun Engn, Dublin 2, Ireland. [Milligan, Michael] Natl Renewable Energy Lab, Golden, CO USA. RP Troy, N (reprint author), Univ Coll Dublin, Sch Elect Elect & Commun Engn, Dublin 2, Ireland. EM niamh.troy@ucd.ie; damian.flynn@ucd.ie; michael.milligan@nrel.gov; mark.oma-lley@ucd.ie OI Flynn, Damian/0000-0003-4638-9333 FU Commission for Energy Regulation; Bord Gais Energy; Bord na Mona Energy; Cylon Controls; EirGrid; Electric Power Research Institute (EPRI); ESB Energy International; ESB Energy Solutions; ESB Networks; Gaelectric; SSE Renewables; Viridian Power Energy; Science Foundation Ireland [06/CP/E005] FX This work was conducted in the Electricity Research Centre, University College Dublin, Ireland, which is supported by the Commission for Energy Regulation, Bord Gais Energy, Bord na Mona Energy, Cylon Controls, EirGrid, the Electric Power Research Institute (EPRI), ESB Energy International, ESB Energy Solutions, ESB Networks, Gaelectric, SSE Renewables, and Viridian Power & Energy. This work was supported by the Science Foundation Ireland under Grant Number 06/CP/E005. Paper no. TPWRS-00980-2011. NR 15 TC 18 Z9 18 U1 0 U2 6 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0885-8950 J9 IEEE T POWER SYST JI IEEE Trans. Power Syst. PD NOV PY 2012 VL 27 IS 4 BP 2196 EP 2205 DI 10.1109/TPWRS.2012.2192141 PG 10 WC Engineering, Electrical & Electronic SC Engineering GA 027YC UT WOS:000310389000049 ER PT J AU Ma, J Makarov, YV Diao, RS Etingov, PV Dagle, JE De Tuglie, E AF Ma, Jian Makarov, Yuri V. Diao, Ruisheng Etingov, Pavel V. Dagle, Jeff E. De Tuglie, Enrico TI The Characteristic Ellipsoid Methodology and its Application in Power Systems SO IEEE TRANSACTIONS ON POWER SYSTEMS LA English DT Article DE Characteristic ellipsoid; decision tree; event detection; minimum volume enclosing ellipsoid; phasor measurement unit; situation awareness; system disturbance ID FAULT DETECTION/LOCATION TECHNIQUE; VOLUME ENCLOSING ELLIPSOIDS; PHASOR MEASUREMENTS; TRANSMISSION-LINES; COMPUTATION; AREA AB The characteristic ellipsoid (CELL) method to monitor dynamic behaviors of a power system is proposed. Multi-dimensional minimum-volume-enclosing characteristic ellipsoids are built using synchronized phasor measurements. System dynamic behaviors are identified by tracking the change rate of the CELL's characteristic indices. Decision tree techniques are used to link the CELL's characteristic indices and the system's dynamic behaviors and to determine types, locations and related information about the dynamic behaviors. The knowledge base of representative transient events is created by offline simulations based on the full Western Electric Coordinating Council (WECC) model. Two case studies demonstrate that the CELL method combined with the decision trees can detect transient events and their features with good accuracy. C1 [Ma, Jian; Makarov, Yuri V.; Diao, Ruisheng; Etingov, Pavel V.; Dagle, Jeff E.] Pacific NW Natl Lab, Richland, WA 99352 USA. [De Tuglie, Enrico] Politecn Bari, Bari, Italy. RP Ma, J (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM jian.ma@pnnl.gov; yuri.makarov@pnnl.gov; ruisheng.diao@pnnl.gov; pavel.etingov@pnnl.gov; jeff.dagle@pnnl.gov; de-tuglie@poliba.it FU U.S. Department of Energy; Lawrence Berkeley National Laboratory; Bonneville Power Administration; North American Electric Reliability Corporation; U.S. Department of Energy through the Consortium for Electric Reliability Technology Solutions; U.S. Department of Energy [DE-AC05-76RL01830] FX The authors would like to thank P. Overholt (the U.S. Department of Energy), J. Eto (Lawrence Berkeley National Laboratory), D. Kosterev (Bonneville Power Administration), and B. Cummings (North American Electric Reliability Corporation) for sponsorship, encouragement, interest, and support of the work. The authors also would like to thank M. Parashar (A. Grid) and M. Varghese (formerly with California Independent System Operator) for the inspiring discussions that ignited the idea of the work. The authors would like to thank N. Moshtagh (University of Pennsylvania) for his help with interpreting the MVEE algorithm, and T. Nguyen, C. Miller, and N. Zhou of PNNL for their contributions on the initial study.; This work was supported by the U.S. Department of Energy through the Consortium for Electric Reliability Technology Solutions. Pacific Northwest National Laboratory (PNNL) is operated by Battelle for the U.S. Department of Energy under Contract DE-AC05-76RL01830. Paper no. TPWRS-01000-2011. NR 21 TC 5 Z9 6 U1 4 U2 16 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0885-8950 J9 IEEE T POWER SYST JI IEEE Trans. Power Syst. PD NOV PY 2012 VL 27 IS 4 BP 2206 EP 2214 DI 10.1109/TPWRS.2012.2195232 PG 9 WC Engineering, Electrical & Electronic SC Engineering GA 027YC UT WOS:000310389000050 ER PT J AU Liu, C Wang, JH Ostrowski, J AF Liu, Cong Wang, Jianhui Ostrowski, James TI Heuristic Prescreening Switchable Branches in Optimal Transmission Switching SO IEEE TRANSACTIONS ON POWER SYSTEMS LA English DT Article DE Mixed integer linear programming; screening; sensitivity factors; transmission switching AB This letter describes the development of a prescreening method to select a few switchable line candidates, effectively reducing the number of integer variables in transmission switching problems. The numerical studies show that the proposed prescreening strategies accelerate identification of high-quality feasible solutions in optimal transmission switching problems. C1 [Liu, Cong; Wang, Jianhui; Ostrowski, James] Argonne Natl Lab, Argonne, IL 60439 USA. [Liu, Cong; Wang, Jianhui; Ostrowski, James] Univ Tennessee, Knoxville, TN 37996 USA. RP Liu, C (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. EM liuc@anl.gov; jianhui.wang@anl.gov; jostrows@utk.edu OI Ostrowski, James/0000-0001-5636-555X FU Office of Electricity Delivery and Energy of U.S. Department of Energy FX Manuscript received September 02, 2011; revised January 23, 2012; accepted March 09, 2012. Date of publication April 27, 2012; date of current version nulldate. This work was supported by the Office of Electricity Delivery and Energy of U.S. Department of Energy. Paper no. PESL-00110-2011. NR 3 TC 21 Z9 21 U1 0 U2 7 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0885-8950 J9 IEEE T POWER SYST JI IEEE Trans. Power Syst. PD NOV PY 2012 VL 27 IS 4 BP 2289 EP 2290 DI 10.1109/TPWRS.2012.2193489 PG 2 WC Engineering, Electrical & Electronic SC Engineering GA 027YC UT WOS:000310389000059 ER PT J AU Squires, RB Noronha, J Hunt, V Garcia-Sastre, A Macken, C Baumgarth, N Suarez, D Pickett, BE Zhang, Y Larsen, CN Ramsey, A Zhou, LW Zaremba, S Kumar, S Deitrich, J Klem, E Scheuermann, RH AF Squires, R. Burke Noronha, Jyothi Hunt, Victoria Garcia-Sastre, Adolfo Macken, Catherine Baumgarth, Nicole Suarez, David Pickett, Brett E. Zhang, Yun Larsen, Christopher N. Ramsey, Alvin Zhou, Liwei Zaremba, Sam Kumar, Sanjeev Deitrich, Jon Klem, Edward Scheuermann, Richard H. TI Influenza Research Database: an integrated bioinformatics resource for influenza research and surveillance SO INFLUENZA AND OTHER RESPIRATORY VIRUSES LA English DT Article DE Bioinformatics; epitope; influenza virus; integrated; surveillance ID MULTIPLE SEQUENCE ALIGNMENT; A VIRUS; EPITOPE DATABASE; HIGH-THROUGHPUT; CELL EPITOPES; MORTALITY; ANTIBODY; INFORMATION; INFECTIONS AB Background The recent emergence of the 2009 pandemic influenza A/H1N1 virus has highlighted the value of free and open access to influenza virus genome sequence data integrated with information about other important virus characteristics. sign The Influenza Research Database (IRD, http://www.fludb.org) is a free, open, publicly-accessible resource funded by the U.S. National Institute of Allergy and Infectious Diseases through the Bioinformatics Resource Centers program. IRD provides a comprehensive, integrated database and analysis resource for influenza sequence, surveillance, and research data, including user-friendly interfaces for data retrieval, visualization and comparative genomics analysis, together with personal log in-protected workbench spaces for saving data sets and analysis results. IRD integrates genomic, proteomic, immune epitope, and surveillance data from a variety of sources, including public databases, computational algorithms, external research groups, and the scientific literature. Results To demonstrate the utility of the data and analysis tools available in IRD, two scientific use cases are presented. A comparison of hemagglutinin sequence conservation and epitope coverage information revealed highly conserved protein regions that can be recognized by the human adaptive immune system as possible targets for inducing cross-protective immunity. Phylogenetic and geospatial analysis of sequences from wild bird surveillance samples revealed a possible evolutionary connection between influenza virus from Delaware Bay shorebirds and Alberta ducks. Conclusions The IRD provides a wealth of integrated data and information about influenza virus to support research of the genetic determinants dictating virus pathogenicity, host range restriction and transmission, and to facilitate development of vaccines, diagnostics, and therapeutics. C1 [Squires, R. Burke; Noronha, Jyothi; Hunt, Victoria; Pickett, Brett E.; Zhang, Yun; Scheuermann, Richard H.] Univ Texas SW Med Ctr Dallas, Dept Pathol, Dallas, TX 75390 USA. [Garcia-Sastre, Adolfo] Mt Sinai Sch Med, Dept Microbiol, New York, NY USA. [Garcia-Sastre, Adolfo] Mt Sinai Sch Med, Dept Med, Div Infect Dis, New York, NY USA. [Garcia-Sastre, Adolfo] Mt Sinai Sch Med, Global Hlth & Emerging Pathogens Inst, New York, NY USA. [Macken, Catherine] Los Alamos Natl Lab, Los Alamos, NM USA. [Baumgarth, Nicole] Univ Calif Davis, Ctr Comparat Med, Davis, CA 95616 USA. [Suarez, David] USDA, SE Poultry Res Lab, Athens, GA USA. [Larsen, Christopher N.; Ramsey, Alvin] Vecna Technol, Greenbelt, MD USA. [Zhou, Liwei; Zaremba, Sam; Kumar, Sanjeev; Deitrich, Jon; Klem, Edward] Hlth IT Syst, Northrop Grumman Informat Syst, Rockville, MD USA. [Scheuermann, Richard H.] Univ Texas SW Med Ctr Dallas, Div Biomed Informat, Dallas, TX 75390 USA. RP Scheuermann, RH (reprint author), Univ Texas SW Med Ctr Dallas, Dept Pathol, 5323 Harry Hines Blvd, Dallas, TX 75390 USA. EM richard.scheuermann@utsouthwestern.edu RI Squires, Richard/A-7163-2008; OI Garcia-Sastre, Adolfo/0000-0002-6551-1827; Scheuermann, Richard/0000-0003-1355-892X; Squires, R Burke/0000-0001-9666-6285 FU NIAID FX First and foremost, we would like to acknowledge the contribution of all providers of data to public database resources like GenBank and IRD. Without their efforts to generate the data and their willingness to make it freely available through public data repositories, the potential for the kind of comprehensive integrative data analysis illustrated here would not be possible. We have especially benefitted from collaborating with the NIAID-funded Centers of Excellence for Influenza Research and Surveillance (CEIRS) who have been extremely helpful in developing data standards, identifying use cases, and sharing their data. We also acknowledge the generous support received from the NIAID - N01AI40041. NR 47 TC 115 Z9 116 U1 3 U2 36 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1750-2640 J9 INFLUENZA OTHER RESP JI Influenza Other Respir. Viruses PD NOV PY 2012 VL 6 IS 6 BP 404 EP 416 DI 10.1111/j.1750-2659.2011.00331.x PG 13 WC Infectious Diseases; Virology SC Infectious Diseases; Virology GA 026IY UT WOS:000310270300021 PM 22260278 ER PT J AU Asgharian, B Price, O McClellan, G Corley, R Einstein, DR Jacob, RE Harkema, J Carey, SA Schelegle, E Hyde, D Kimbell, JS Miller, FJ AF Asgharian, Bahman Price, Owen McClellan, Gene Corley, Rick Einstein, Daniel R. Jacob, Richard E. Harkema, Jack Carey, Stephan A. Schelegle, Edward Hyde, Dallas Kimbell, Julia S. Miller, Frederick J. TI Development of a rhesus monkey lung geometry model and application to particle deposition in comparison to humans SO INHALATION TOXICOLOGY LA English DT Article DE Rhesus monkeys; lung geometry; breathing parameters; particles; deposition modeling; humans ID MULTIPLE-PATH MODEL; AEROSOL DEPOSITION; NASAL AIRWAYS; AIR-FLOW; VENTILATION; RAT; DISEASE; CASTS; TREE AB The exposure-dose-response characterization of an inhalation hazard established in an animal species needs to be translated to an equivalent characterization in humans relative to comparable doses or exposure scenarios. Here, the first geometry model of the conducting airways for rhesus monkeys is developed based upon CT images of the conducting airways of a 6-month-old male, rhesus monkey. An algorithm was developed for adding the alveolar region airways using published rhesus morphometric data. The resultant lung geometry model can be used in mechanistic particle or gaseous dosimetry models. Such dosimetry models require estimates of the upper respiratory tract volume of the animal and the functional residual capacity, as well as of the tidal volume and breathing frequency of the animal. The relationship of these variables to rhesus monkeys of differing body weights was established by synthesizing and modeling published data as well as modeling pulmonary function measurements on 121 rhesus control animals. Deposition patterns of particles up to 10 mu m in size were examined for endotracheal and and up to 5 mu m for spontaneous breathing in infant and young adult monkeys and compared to those for humans. Deposition fraction of respirable size particles was found to be higher in the conducting airways of infant and young adult rhesus monkeys compared to humans. Due to the filtering effect of the conducting airways, pulmonary deposition in rhesus monkeys was lower than that in humans. Future research areas are identified that would either allow replacing assumptions or improving the newly developed lung model. C1 [Asgharian, Bahman] Appl Res Associates Inc, Raleigh, NC 27615 USA. [Price, Owen; McClellan, Gene] Appl Res Associates Inc, Arlington, VA 22203 USA. [Corley, Rick; Einstein, Daniel R.; Jacob, Richard E.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Harkema, Jack] Michigan State Univ, Coll Vet Med, Dept Pathobiol & Diagnost Invest, E Lansing, MI 48824 USA. [Carey, Stephan A.] Michigan State Univ, Coll Vet Med, Dept Small Anim Clin Sci, E Lansing, MI 48824 USA. [Schelegle, Edward; Hyde, Dallas] Univ Calif Davis, Sch Vet Med, Davis, CA 95616 USA. [Hyde, Dallas] Univ Calif Davis, Calif Natl Primate Res Ctr, Davis, CA 95616 USA. [Kimbell, Julia S.] Univ N Carolina, Sch Med, Dept Otolaryngol Head & Neck Surg, Chapel Hill, NC 27599 USA. [Miller, Frederick J.] Fred J Miller & Associates LLC, Cary, NC 27511 USA. RP Asgharian, B (reprint author), Appl Res Associates Inc, 8537 6 Forks Rd,Suite 600, Raleigh, NC 27615 USA. EM basgharian@ara.com FU Defense Threat Reduction Agency [DTRA01-03-D-0014-0030]; NIH [P01 ES011617]; National Heart, Lung, and Blood Institute [NHLBI R01 HL073598]; National Institute of Environmental Health Sciences of the National Institutes of Health [NIEHS P01 ES011617]; Department of Energy's Office of Biological and Environmental Research FX This work was funded in part by the Defense Threat Reduction Agency via contract DTRA01-03-D-0014-0030. Nasal airway imaging and geometries were supported by funding from NIH P01 ES011617. All imaging, image processing, and lung geometry data acquisition was supported by grants from the National Heart, Lung, and Blood Institute (NHLBI R01 HL073598) and the National Institute of Environmental Health Sciences (NIEHS P01 ES011617) of the National Institutes of Health. A portion of this research was performed using EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. The authors declare that they have no financial interest in the findings of this study. NR 53 TC 10 Z9 10 U1 1 U2 10 PU INFORMA HEALTHCARE PI LONDON PA TELEPHONE HOUSE, 69-77 PAUL STREET, LONDON EC2A 4LQ, ENGLAND SN 0895-8378 J9 INHAL TOXICOL JI Inhal. Toxicol. PD NOV PY 2012 VL 24 IS 13 BP 869 EP 899 DI 10.3109/08958378.2012.725782 PG 31 WC Toxicology SC Toxicology GA 032HV UT WOS:000310707300001 PM 23121298 ER PT J AU Hagos, S Leung, LR AF Hagos, Samson Leung, L. Ruby TI Large-scale environmental variables and transition to deep convection in cloud resolving model simulations: A vector representation SO JOURNAL OF ADVANCES IN MODELING EARTH SYSTEMS LA English DT Article ID SHALLOW; SENSITIVITY; RESOLUTION; LAND; TOP AB Cloud resolving model simulations and vector analysis are used to develop a quantitative method of assessing regional variations in the relationships between various large-scale environmental variables and the transition to deep convection. Results of the CRM simulations from three tropical regions are used to cluster environmental conditions under which transition to deep convection does and does not take place. Projections of the large-scale environmental variables on the difference between these two clusters are used to quantify the roles of these variables in the transition to deep convection. While the transition to deep convection is most sensitive to moisture and vertical velocity perturbations, the details of the profiles of the anomalies vary from region to region. In comparison, the transition to deep convection is found to be much less sensitive to temperature anomalies over all three regions. The vector formulation presented in this study represents a simple general framework for quantifying various aspects of how the transition to deep convection is sensitive to environmental conditions. C1 [Hagos, Samson; Leung, L. Ruby] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Hagos, S (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM samson.hagos@pnl.gov RI hagos, samson /K-5556-2012 FU U.S. Department of Energy under the Atmospheric Systems Research Program; U.S. Department of Energy [DE-AC06-76RLO1830] FX The authors thank William I. Gustafson Jr. for his comments and suggestions. The TWP-ICE best estimate forcing data was provided by Christian Jakob. This work is supported by the U.S. Department of Energy under the Atmospheric Systems Research Program. Computing resources for the simulations are provided by the National Center for Computational Sciences (NCCS) through the INCITE Climate End Station project and National Energy Research Scientific Computing Center (NERSC). Pacific Northwest National Laboratory is operated by Battelle for the U.S. Department of Energy under contract DE-AC06-76RLO1830. NR 20 TC 0 Z9 0 U1 1 U2 9 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 1942-2466 J9 J ADV MODEL EARTH SY JI J. Adv. Model. Earth Syst. PD NOV 1 PY 2012 VL 4 AR M11001 DI 10.1029/2012MS000155 PG 11 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 032DS UT WOS:000310693000001 ER PT J AU Florea, RS Hubbard, CR Solanki, KN Bammann, DJ Whittington, WR Marin, EB AF Florea, R. S. Hubbard, C. R. Solanki, K. N. Bammann, D. J. Whittington, W. R. Marin, E. B. TI Quantifying residual stresses in resistance spot welding of 6061-T6 aluminum alloy sheets via neutron diffraction measurements SO JOURNAL OF MATERIALS PROCESSING TECHNOLOGY LA English DT Article DE Resistance spot welding; Aluminum alloy; Neutron diffraction; Residual stress mapping; Electron backscatter diffraction; Optical microscopy; Quasi-static testing ID MECHANICAL-PROPERTIES; PART 1; STEEL; MICROSTRUCTURE AB Residual strains of resistance spot welded joints of 6061-T6 aluminum alloy sheets were measured in three different directions denoted as in-plane longitudinal (sigma(11)) in-plane transversal (sigma(22)), and normal (sigma(33)). The welding process parameters were established to meet or exceed MIL-W-6858D specifications (i.e., approximately 5.7 mm weld nugget and minimum shearing force of 3.8 kN per weld confirmed via quasi-static tensile testing). Electron backscatter diffraction (EBSD) and optical microscopy (OM) were performed to determine grain size and orientation. The residual stress measurements were taken at a series of points along the weld centerline at depths corresponding to the weld mid-plane and at both 1 mm below the top surface of the plate and 1 mm above bottom surface. The residual stresses were captured on the fusion zone (FZ), heat affected zone (HAZ) and base metal (BM) of the resistance spot welded joint. Neutron diffraction results show residual stresses in the weld are approximately 40% lower than yield strength of the parent material. The maximum variation in residual stresses occurs, as expected, in the vertical position of the specimen because of the orientation of electrode clamping forces that produce a non-uniform solidification pattern. Despite the high anisotropy of the welding nugget and surrounding area, a significant result is that sigma(33) measured stress values are negligible in both the horizontal and vertical directions of the specimen. Consequently, microstructure-property relationships characterized here can indeed inform continuum material models for application in multiscale models. (C) 2012 Elsevier B.V. All rights reserved. C1 [Florea, R. S.; Bammann, D. J.; Whittington, W. R.] Mississippi State Univ, Dept Mech Engn, Mississippi State, MS 39762 USA. [Florea, R. S.; Bammann, D. J.; Whittington, W. R.; Marin, E. B.] Ctr Adv Vehicular Syst, Starkville, MS 39759 USA. [Hubbard, C. R.] Oak Ridge Natl Lab, High Temp Mat Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Solanki, K. N.] Arizona State Univ, Sch Engn Matter Transport & Energy, Tempe, AZ 85287 USA. RP Florea, RS (reprint author), Mississippi State Univ, Dept Mech Engn, Mail Stop 9552,210 Carpenter Bldg, Mississippi State, MS 39762 USA. EM rf2@msstate.edu RI Solanki, Kiran/E-8337-2010; OI Solanki, Kiran/0000-0002-4385-620X FU Center of Advanced Vehicular Systems (CAVS); U.S. Army-TARDEC; U.S. Army TACOM Life Cycle Command [W56HZV-08-C-0236]; Mississippi State University; Department of Energy; DOE-EERE-Vehicle Technologies; DOE-OS Facilities Division FX The authors would like to thank the Center of Advanced Vehicular Systems (CAVS) and the U.S. Army-TARDEC for supporting this work. This material is based upon work supported by the U.S. Army TACOM Life Cycle Command under Contract No. W56HZV-08-C-0236, through a subcontract with Mississippi State University, and it was performed for the Simulation Based Reliability and Safety (SimBRS) research program. Any opinions, findings and conclusions or recommendations expressed in this material are those of the author(s) and do not necessarily reflect the views of the U.S. Army TACOM Life Cycle Command.; Oak Ridge National Laboratory, High Temperature Materials User Facility which is sponsored by the Department of Energy, Energy Efficiency and Renewable Energy, Transportation Program provided the opportunity to use the neutron facilities required for this work. HTML is sponsored by DOE-EERE-Vehicle Technologies and HFIR by DOE-OS Facilities Division. NR 21 TC 6 Z9 7 U1 4 U2 28 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0924-0136 J9 J MATER PROCESS TECH JI J. Mater. Process. Technol. PD NOV PY 2012 VL 212 IS 11 BP 2358 EP 2370 DI 10.1016/j.jmatprotec.2012.06.024 PG 13 WC Engineering, Industrial; Engineering, Manufacturing; Materials Science, Multidisciplinary SC Engineering; Materials Science GA 017DD UT WOS:000309569400021 ER PT J AU Yoon, WS Nam, KW Jang, D Chung, KY Hanson, J Chen, JM Yang, XQ AF Yoon, Won-Sub Nam, Kyung-Wan Jang, Donghyuk Chung, Kyung Yoon Hanson, Jonathan Chen, Jin-Ming Yang, Xiao-Qing TI Structural study of the coating effect on the thermal stability of charged MgO-coated LiNi0.8Co0.2O2 cathodes investigated by in situ XRD SO JOURNAL OF POWER SOURCES LA English DT Article DE Lithium battery; Thermal stability; MgO coating; In situ XRD; Layered compounds ID LI-ION BATTERIES; TIME-RESOLVED XRD; DIFFERENTIAL SCANNING CALORIMETRY; LICOO2 CATHODE; DECOMPOSITION; IMPROVEMENT; OXIDE; CELL AB Safety concerns in high-performance lithium rechargeable batteries are one of the major technical barriers that have to be overcome for successful commercialization of more demanding applications like electric vehicles and electric energy storage for renewable energy sources. The thermal stability of the charged cathode materials is critical in the safety characteristics of Li batteries, which is related to the occurrence of exothermic reactions in charged batteries at elevated temperatures that ultimately result in thermal runaway and catastrophic failure of the battery. The thermal runaway has been attributed to the reactions between the charged electrodes and the electrolyte. Therefore, in-depth understanding of the structural changes of the charged cathode material during thermal decomposition reactions, with or without the presence of electrolytes and their relationship with the thermal stability of the cathode material is very important. One of the effective ways to improve the thermal stability of charged cathodes is to modify the electrode materials' surface by coating with stable metal oxides. Here we report the effect of surface modification on the structural changes and their relationship with thermal stability of charged MgO-coated LiNi0.8Co0.2O2 cathodes by using in situ XRD technique in a wide temperature range from 25 degrees C to 450 degrees C with and without the presence of electrolyte in comparison with bare LiNi0.8Co0.2O2 cathodes. (C) 2012 Elsevier B.V. All rights reserved. C1 [Yoon, Won-Sub; Jang, Donghyuk] Sungkyunkwan Univ, Dept Energy Sci, Suwon 440746, South Korea. [Nam, Kyung-Wan; Hanson, Jonathan; Yang, Xiao-Qing] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Chung, Kyung Yoon] Korea Inst Sci & Technol, Ctr Energy Convergence, Seoul 136791, South Korea. [Chen, Jin-Ming] Ind Technol Res Inst, Mat Res Labs, Hsinchu 310, Taiwan. RP Yoon, WS (reprint author), Sungkyunkwan Univ, Dept Energy Sci, Suwon 440746, South Korea. EM wsyoon@gmail.com RI Yoon, Won-Sub/H-2343-2011; Nam, Kyung-Wan/B-9029-2013; Nam, Kyung-Wan/E-9063-2015; Chung, Kyung Yoon/E-4646-2011 OI Nam, Kyung-Wan/0000-0001-6278-6369; Nam, Kyung-Wan/0000-0001-6278-6369; Chung, Kyung Yoon/0000-0002-1273-746X FU U.S. Department of Energy, Office of Vehicle Technologies [DEAC02-98CH10886]; Global Research Laboratory Program through the National Research Foundation of Korea (NRF); Ministry of Education, Science and Technology (MEST) [2011-00115]; National Research Foundation; Fundamental R&D Program for Technology of World Premier Materials; Korean Government [NRF-2010-C1AAA001-2010-0029065/2009-0067121/R31-2008-10029] FX The work done at Brookhaven National Lab, was supported by the U.S. Department of Energy, the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies under Contract Number DEAC02-98CH10886. The work done at KIST was supported by the Global Research Laboratory Program through the National Research Foundation of Korea (NRF), which is funded by the Ministry of Education, Science and Technology (MEST) (grant number: 2011-00115). The work at Sungkyunkwan University was supported by the National Research Foundation and the Fundamental R&D Program for Technology of World Premier Materials funded by the Korean Government (NRF-2010-C1AAA001-2010-0029065/2009-0067121/R31-2008-10029). NR 25 TC 17 Z9 21 U1 11 U2 132 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 J9 J POWER SOURCES JI J. Power Sources PD NOV 1 PY 2012 VL 217 BP 128 EP 134 DI 10.1016/j.jpowsour.2012.05.028 PG 7 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA 005XA UT WOS:000308782200021 ER PT J AU Corpuz, AR Olson, TS Joghee, P Pylypenko, S Dameron, AA Dinh, HN O'Neill, KJ Hurst, KE Bender, G Gennett, T Pivovar, BS Richards, RM O'Hayre, RP AF Corpuz, A. R. Olson, T. S. Joghee, P. Pylypenko, S. Dameron, A. A. Dinh, H. N. O'Neill, K. J. Hurst, K. E. Bender, G. Gennett, T. Pivovar, B. S. Richards, R. M. O'Hayre, R. P. TI Effect of a nitrogen-doped PtRu/carbon anode catalyst on the durability of a direct methanol fuel cell SO JOURNAL OF POWER SOURCES LA English DT Article DE Nitrogen doping; Fuel cell; Membrane electrode assembly; Platinum ruthenium; Durability; Anode ID OXYGEN REDUCTION REACTION; PLATINUM NANOPARTICLES; CARBON NANOTUBES; SUPPORT STRUCTURES; POROUS CARBON; CNX NANOTUBES; PERFORMANCE; ELECTROCATALYSTS; OXIDATION; CROSSOVER AB Electrochemical performance and durability of PtRu supported on N-doped Vulcan is evaluated as an anode in membrane electrode assembly (MEA) single-cell direct methanol fuel cell (DMFC) studies. This material is compared to two reference materials, an in-house PtRu catalyst supported on undoped Vulcan, prepared under the same conditions as the N-doped material besides doping, and a commercial PtRu/C (JM5000). Durability was tested out to 645 h, with periodic interruption for electrochemical testing. After durability, the MEA with N-doped PtRu/C retained more electrochemically active metal on the anode than the MEAs with commercial PtRu/C and undoped PtRu/C (124 compared to 106 and 82 cm(2) anode active area per cm(2) geometric surface area, respectively). From cathode CO stripping experiments and SEM-EDS studies, it was determined that the MEA with the undoped PtRu/C anode has twice as much ruthenium crossover as the MEA with the N-doped PtRu/C anode. Overall, the MEA with N-doped PtRu/C demonstrates significantly better methanol:air polarization performance compared to the MEA with undoped PtRu/C, and performs comparably to the MEA made with the commercial PtRu/C. The increase in durability for the MEA with the N-doped anode is attributed to nitrogen doping mitigating both anode metal dissolution and Ru crossover. (C) 2012 Elsevier By. All rights reserved. C1 [Corpuz, A. R.; Richards, R. M.] Colorado Sch Mines, Dept Chem, Golden, CO 80401 USA. [Olson, T. S.; Dameron, A. A.; Dinh, H. N.; O'Neill, K. J.; Hurst, K. E.; Bender, G.; Gennett, T.; Pivovar, B. S.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Joghee, P.; Pylypenko, S.; O'Hayre, R. P.] Colorado Sch Mines, Dept Met & Mat Engn, Golden, CO 80401 USA. RP Corpuz, AR (reprint author), Colorado Sch Mines, Dept Chem, 1500 Illinois St, Golden, CO 80401 USA. EM april.corpuz@gmail.com RI O'Hayre, Ryan/A-8183-2009; Richards, Ryan/B-3513-2008 FU Army Research Office [W911NF-09-1-0528]; U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, and Office of Basic Energy Science [DE-AC36-08-GO28308] FX Work at CSM supported by the Army Research Office under grant #W911NF-09-1-0528. Work at the National Renewable Energy Laboratory (NREL) was supported by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, and Office of Basic Energy Science, under Contract No. DE-AC36-08-GO28308. NR 45 TC 23 Z9 23 U1 1 U2 98 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 J9 J POWER SOURCES JI J. Power Sources PD NOV 1 PY 2012 VL 217 BP 142 EP 151 DI 10.1016/j.jpowsour.2012.06.012 PG 10 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA 005XA UT WOS:000308782200023 ER PT J AU Zheng, HH Zhang, L Liu, G Song, XY Battaglia, VS AF Zheng, Honghe Zhang, Li Liu, Gao Song, Xiangyun Battaglia, Vincent S. TI Correlationship between electrode mechanics and long-term cycling performance for graphite anode in lithium ion cells SO JOURNAL OF POWER SOURCES LA English DT Article DE Lithium ion batteries; Graphite anode; Mechanical properties; Cycle life ID NUMERICAL-SIMULATION; BATTERIES; PARTICLES; INSERTION; CATHODE; INTERCALATION; BINDER AB In the development of lithium ion batteries for electric vehicle applications, much effort has been made in fabrication and optimization of active materials. Mechanical properties of the electrode laminate, which are also very critical determining the durability of the cell, have long been ignored. In this study, graphite laminates of the same chemical composition are prepared by using different mixing technologies. With similar breaking strength, Young's modulus of the laminate is found to be very different according to the mixing order. Electrochemical performances of the graphite laminates are investigated against Li anode and Li[Ni1/3Co1/3Mn1/3]O-2 cathode, respectively. Long-term cycling performance is closely related with the Young's modulus of the graphite laminate. Whereas the laminates of low modulus cycles well during the investigated 600 deep charge-discharge cycles, the electrodes of high modulus fail at around 350 cycles. Electrochemical degradation mechanism for the laminate of high modulus is associated with the significant impedance rise aroused from mechanical failure. After the long-term cycling test, lots of cracks are observed on the high modulus electrode along the particle boundaries while the mechanical integrity of the low modulus laminate is well maintained. (C) 2012 Elsevier B.V. All rights reserved. C1 [Zheng, Honghe; Zhang, Li] Suzhou Univ, Sch Energy, Suzhou 215006, Jiangsu, Peoples R China. [Zheng, Honghe; Liu, Gao; Song, Xiangyun; Battaglia, Vincent S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Zheng, HH (reprint author), Suzhou Univ, Sch Energy, Suzhou 215006, Jiangsu, Peoples R China. EM hhzheng66@yahoo.com.cn FU Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy [DE-AC02-05CH11231]; Natural Science Foundation of China [NSFC 21073129] FX This work was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231 and the Natural Science Foundation of China (NSFC 21073129). NR 30 TC 23 Z9 25 U1 4 U2 129 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 J9 J POWER SOURCES JI J. Power Sources PD NOV 1 PY 2012 VL 217 BP 530 EP 537 DI 10.1016/j.jpowsour.2012.06.045 PG 8 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA 005XA UT WOS:000308782200077 ER PT J AU Smith, DF Kharchenko, A Konijnenburg, M Klinkert, I Pasa-Tolic, L Heeren, RMA AF Smith, Donald F. Kharchenko, Andriy Konijnenburg, Marco Klinkert, Ivo Pasa-Tolic, Ljiljana Heeren, Ron M. A. TI Advanced Mass Calibration and Visualization for FT-ICR Mass Spectrometry Imaging SO JOURNAL OF THE AMERICAN SOCIETY FOR MASS SPECTROMETRY LA English DT Article DE Imaging mass spectrometry; Lipids; FT-MS; Fourier transform; High resolution ID CYCLOTRON RESONANCE FREQUENCIES; MULTIPLE LINEAR-REGRESSION; SPACE-CHARGE; HIGH-RESOLUTION; ACCURACY; TISSUE; FTICR; MS; PEPTIDES; IONS AB Mass spectrometry imaging by Fourier transform ion cyclotron resonance (FT-ICR) yields hundreds of unique peaks, many of which cannot be resolved by lower performance mass spectrometers. The high mass accuracy and high mass resolving power allow confident identification of small molecules and lipids directly from biological tissue sections. Here, calibration strategies for FT-ICR MS imaging were investigated. Sub-parts-per-million mass accuracy is demonstrated over an entire tissue section. Ion abundance fluctuations are corrected by addition of total and relative ion abundances for a root-mean-square error of 0.158 ppm on 16,764 peaks. A new approach for visualization of FT-ICR MS imaging data at high resolution is presented. The "Mosaic Datacube" provides a flexible means to visualize the entire mass range at a mass spectral bin width of 0.001 Da. The high resolution Mosaic Datacube resolves spectral features not visible at lower bin widths, while retaining the high mass accuracy from the calibration methods discussed. C1 [Smith, Donald F.; Kharchenko, Andriy; Konijnenburg, Marco; Klinkert, Ivo; Heeren, Ron M. A.] FOM Inst AMOLF, NL-1098 XG Amsterdam, Netherlands. [Smith, Donald F.; Pasa-Tolic, Ljiljana] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. RP Heeren, RMA (reprint author), FOM Inst AMOLF, Sci Pk 104, NL-1098 XG Amsterdam, Netherlands. EM heeren@amolf.nl RI Smith, Donald/K-3939-2013; OI Heeren, Ron/0000-0002-6533-7179 FU Dutch national program COMMIT; American Reinvestment and Recovery Act of 2009; U.S. Department of Energy (DOE) Office of Biological and Environmental Research; Department of Energy's Office of Biological and Environmental Research; U.S. Department of Energy [DE-AC05-76RLO 1830] FX This work is part of the research program of the Foundation for Fundamental Research on Matter (FOM), which is part of The Netherlands Organization for Scientific Research (NWO). This publication was supported by the Dutch national program COMMIT. Portions of this research were supported by the American Reinvestment and Recovery Act of 2009 and the U.S. Department of Energy (DOE) Office of Biological and Environmental Research. The research described in this article was performed at the W. R. Wiley Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory (PNNL). PNNL is operated by Battelle for the U.S. Department of Energy under contract DE-AC05-76RLO 1830. The authors thank Si Wu for supplying the oligosaccharide standard, Nikola Tolic for help with the lock mass calibration, and Julia Jungmann for assistance in debugging the Matlab code. NR 39 TC 15 Z9 15 U1 0 U2 27 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1044-0305 J9 J AM SOC MASS SPECTR JI J. Am. Soc. Mass Spectrom. PD NOV PY 2012 VL 23 IS 11 BP 1865 EP 1872 DI 10.1007/s13361-012-0464-1 PG 8 WC Biochemical Research Methods; Chemistry, Analytical; Chemistry, Physical; Spectroscopy SC Biochemistry & Molecular Biology; Chemistry; Spectroscopy GA 022FS UT WOS:000309941700004 PM 22926971 ER PT J AU Marchese, R Grandori, R Carloni, P Raugei, S AF Marchese, Roberto Grandori, Rita Carloni, Paolo Raugei, Simone TI A Computational Model for Protein Ionization by Electrospray Based on Gas-Phase Basicity SO JOURNAL OF THE AMERICAN SOCIETY FOR MASS SPECTROMETRY LA English DT Article DE Electrospray ionization; Protein ionization; Gas-phase basicity; Monte-Carlo sampling; Molecular-dynamics; Simulations; Density functional theory calculations ID CHARGE-STATE DISTRIBUTIONS; MASS-SPECTROMETRY; SURFACE-TENSION; AB-INITIO; ESI-MS; DENSITY; IONS; SIMULATION; COMPLEXES; MECHANISM AB Identifying the key factor(s) governing the overall protein charge is crucial for the interpretation of electrospray-ionization mass spectrometry data. Current hypotheses invoke different principles for folded and unfolded proteins. Here, first we investigate the gas-phase structure and energetics of several proteins of variable size and different folds. The conformer and protomer space of these proteins ions is explored exhaustively by hybrid Monte-Carlo/molecular dynamics calculations, allowing for zwitterionic states. From these calculations, the apparent gas-phase basicity of desolvated protein ions turns out to be the unifying trait dictating protein ionization by electrospray. Next, we develop a simple, general, adjustable-parameter-free model for the potential energy function of proteins. The model is capable to predict with remarkable accuracy the experimental charge of folded proteins and its well-known correlation with the square root of protein mass. C1 [Grandori, Rita] Univ Milano Bicocca, Dept Biotechnol & Biosci, Milan, Italy. [Marchese, Roberto] SISSA, I-34014 Trieste, Italy. [Marchese, Roberto] INFM DEMOCRITOS Ctr, I-34014 Trieste, Italy. [Carloni, Paolo; Raugei, Simone] German Res Sch Simulat Sci, D-52425 Julich, Germany. [Carloni, Paolo; Raugei, Simone] Forschungszentrum Julich, Inst Adv Simulat IAS 5, D-52425 Julich, Germany. [Raugei, Simone] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. RP Grandori, R (reprint author), Univ Milano Bicocca, Dept Biotechnol & Biosci, Milan, Italy. EM rita.grandori@unimib.it; simone.raugei@pnnl.gov RI Carloni, Paolo/H-8736-2013 NR 52 TC 13 Z9 13 U1 3 U2 31 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1044-0305 J9 J AM SOC MASS SPECTR JI J. Am. Soc. Mass Spectrom. PD NOV PY 2012 VL 23 IS 11 BP 1903 EP 1910 DI 10.1007/s13361-012-0449-0 PG 8 WC Biochemical Research Methods; Chemistry, Analytical; Chemistry, Physical; Spectroscopy SC Biochemistry & Molecular Biology; Chemistry; Spectroscopy GA 022FS UT WOS:000309941700008 PM 22993040 ER PT J AU Guimond, SR Reisner, JM AF Guimond, Stephen R. Reisner, Jon M. TI A Latent Heat Retrieval and Its Effects on the Intensity and Structure Change of Hurricane Guillermo (1997). Part II: Numerical Simulations SO JOURNAL OF THE ATMOSPHERIC SCIENCES LA English DT Article ID TROPICAL CYCLONES; MICROPHYSICAL PROCESSES; MODEL SIMULATIONS; DATA ASSIMILATION; MESOSCALE MODEL; SENSITIVITY; PREDICTION; EVOLUTION; FIELDS; IMPACT AB In Part I of this study, a new algorithm for retrieving the latent heat field in tropical cyclones from airborne Doppler radar was presented and fields from rapidly intensifying Hurricane Guillermo (1997) were shown. In Part II, the usefulness and relative accuracy of the retrievals is assessed by inserting the heating into realistic numerical simulations at 2-km resolution and comparing the generated wind structure to the radar analyses of Guillermo. Results show that using the latent heat retrievals as forcing produces very low intensity and structure errors (in terms of tangential wind speed errors and explained wind variance) and significantly improves simulations relative to a predictive run that is highly calibrated to the latent heat retrievals by using an ensemble Kalman filter procedure to estimate values of key model parameters. Releasing all the heating/cooling in the latent heat retrieval results in a simulation with a large positive bias in Guillermo's intensity that motivates the need to determine the saturation state in the hurricane inner-core retrieval through a procedure similar to that described in Part I of this study. The heating retrievals accomplish high-quality structure statistics by forcing asymmetries in the wind field with the generally correct amplitude, placement, and timing. In contrast, the latent heating fields generated in the predictive simulation contain a significant bias toward large values and are concentrated in bands (rather than discrete cells) stretched around the vortex. The Doppler radar based latent heat retrievals presented in this series of papers should prove useful for convection initialization and data assimilation to reduce errors in numerical simulations of tropical cyclones. C1 [Guimond, Stephen R.] Florida State Univ, Ctr Ocean Atmospher Predict Studies, Tallahassee, FL 32306 USA. [Guimond, Stephen R.] Florida State Univ, Dept Earth Ocean & Atmospher Sci, Tallahassee, FL 32306 USA. [Reisner, Jon M.] Los Alamos Natl Lab, Los Alamos, NM USA. RP Guimond, SR (reprint author), NASA, Goddard Space Flight Ctr, Code 612, Greenbelt, MD 20771 USA. EM stephen.guimond@nasa.gov FU Los Alamos National Laboratory; NASA; NOAA FX The first author would like to thank Dr. Paul Reasor and Dr. Matt Eastin for providing their Doppler radar analysis of Guillermo. Thanks go to Dr. Mark Bourassa and Dr. Robert Hart for several discussions on the work and for their useful suggestions. Dr. Humberto Godinez is acknowledged for providing the parameter estimates and output from his EnKF work. Dr. Jason Sippel and Dr. Gerald Heymsfield also provided some helpful comments. In addition, we thank all of the reviewers for their constructive criticism. This research was supported by the Los Alamos National Laboratory through a project entitled "Flash Before the Storm: Predicting Hurricane Intensification Using LANL Lightning Data" with Dr. Chris Jeffery, the PI. Financial support was also provided by a NASA ocean vector winds contract and a NOAA grant to Dr. Mark Bourassa. NR 31 TC 1 Z9 1 U1 2 U2 3 PU AMER METEOROLOGICAL SOC PI BOSTON PA 45 BEACON ST, BOSTON, MA 02108-3693 USA SN 0022-4928 J9 J ATMOS SCI JI J. Atmos. Sci. PD NOV PY 2012 VL 69 IS 11 BP 3128 EP 3146 DI 10.1175/JAS-D-11-0201.1 PG 19 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 031OU UT WOS:000310652500003 ER PT J AU Godinez, HC Reisner, JM Fierro, AO Guimond, SR Kao, J AF Godinez, Humberto C. Reisner, Jon M. Fierro, Alexandre O. Guimond, Stephen R. Kao, Jim TI Determining Key Model Parameters of Rapidly Intensifying Hurricane Guillermo (1997) Using the Ensemble Kalman Filter SO JOURNAL OF THE ATMOSPHERIC SCIENCES LA English DT Article ID QUASI-GEOSTROPHIC MODEL; DATA ASSIMILATION; RADAR OBSERVATIONS; FIELDS; STATE AB In this work the authors determine key model parameters for rapidly intensifying Hurricane Guillermo (1997) using the ensemble Kalman filter (EnKF). The approach is to utilize the EnKF as a tool only to estimate the parameter values of the model for a particular dataset. The assimilation is performed using dual-Doppler radar observations obtained during the period of rapid intensification of Hurricane Guillermo. A unique aspect of Guillermo was that during the period of radar observations strong convective bursts, attributable to wind shear, formed primarily within the eastern semicircle of the eyewall. To reproduce this observed structure within a hurricane model, background wind shear of some magnitude must be specified and turbulence and surface parameters appropriately specified so that the impact of the shear on the simulated hurricane vortex can be realized. To identify the complex nonlinear interactions induced by changes in these parameters, an ensemble of model simulations have been conducted in which individual members were formulated by sampling the parameters within a certain range via a Latin hypercube approach. The ensemble and the data, derived latent heat and horizontal winds from the dual-Doppler radar observations, are utilized in the EnKF to obtain varying estimates of the model parameters. The parameters are estimated at each time instance, and a final parameter value is obtained by computing the average overtime. Individual simulations were conducted using the estimates, with the simulation using latent heat parameter estimates producing the lowest overall model forecast error. C1 [Godinez, Humberto C.; Fierro, Alexandre O.] Los Alamos Natl Lab, Space & Remote Sensing Grp, Earth & Environm Sci Div, Los Alamos, NM 87545 USA. [Fierro, Alexandre O.] NOAA, Cooperat Inst Mesoscale Meteorol Studies, Norman, OK USA. [Guimond, Stephen R.] Florida State Univ, Ctr Ocean Atmospher Predict Studies, Tallahassee, FL 32306 USA. RP Godinez, HC (reprint author), Los Alamos Natl Lab, Space & Remote Sensing Grp, Earth & Environm Sci Div, MS B284, Los Alamos, NM 87545 USA. EM hgodinez@lanl.gov RI Fierro, Alexandre/C-4733-2014 OI Fierro, Alexandre/0000-0002-4859-1255 FU National Nuclear Security Administration of the U.S. Department of Energy under DOE [W-7405-ENG-36, LA-UR-10-04291]; Laboratory Directed Research and Development Program of the Los Alamos National Laboratory FX This work was supported by the Laboratory Directed Research and Development Program of the Los Alamos National Laboratory, which is under the auspices of the National Nuclear Security Administration of the U.S. Department of Energy under DOE Contracts W-7405-ENG-36 and LA-UR-10-04291. Computer resources were provided both by the Computing Division at Los Alamos and the Oak Ridge National Laboratory Cray clusters; approved for public release, LA-UR-11-10121. NR 30 TC 6 Z9 6 U1 0 U2 6 PU AMER METEOROLOGICAL SOC PI BOSTON PA 45 BEACON ST, BOSTON, MA 02108-3693 USA SN 0022-4928 J9 J ATMOS SCI JI J. Atmos. Sci. PD NOV PY 2012 VL 69 IS 11 BP 3147 EP 3171 DI 10.1175/JAS-D-12-022.1 PG 25 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA 031OU UT WOS:000310652500004 ER PT J AU Beasley, JC Rhodes, OE AF Beasley, James C. Rhodes, Olin E. TI Are raccoons limited by the availability of breeding resources? Evidence of variability in fecundity at fine spatial scales SO JOURNAL OF WILDLIFE MANAGEMENT LA English DT Article DE age structure; carnivore; demography; fragmentation; mesopredator; nest predation; placental scars; population dynamics; Procyon lotor; rabies ID AGE-SPECIFIC REPRODUCTION; PROCYON-LOTOR; NORTHERN INDIANA; DEN SELECTION; POPULATION; LANDSCAPES; ATTRIBUTES; FRAGMENTATION; PERFORMANCE; PATTERNS AB Despite their behavioral plasticity, recent research suggests raccoons (Procyon lotor) exhibit variability in demography and genetic structure among individual habitat patches in landscapes heavily affected by anthropogenic land use. Consequently, elucidation of vital rates at fine-spatial scales is needed to implement appropriate management strategies for this species. To evaluate the degree of variability in productivity that exists among individual habitat patches, we collected reproductive (n?=?170) and cementum annuli age data (n?=?383) for raccoons occupying 30 forest patches varying in local and landscape-level habitat attributes within a highly fragmented agricultural ecosystem. Across all females sampled, pregnancy rates averaged 85% but were highly variable among ages (range: 47100%). Average litter sizes ranged from 3.2 to 4.7, but did not differ as a function of age. At the landscape-level, we observed significant variability among habitat patches in the total number of offspring produced (range: 080), indicating that individual patches vary in their contribution to the overall size and stability of the global (landscape-level) population. Variability in productivity among habitat patches primarily was driven by local differences in the availability of denning resources, likely because of the influence of this variable on variability in the number, age structure, and reproductive rate of females. Our results suggest that in agricultural ecosystems, the reproductive potential and temporal stability of raccoons within individual habitat fragments is inextricably linked to the density of tree cavities. (c) 2012 The Wildlife Society. C1 [Beasley, James C.; Rhodes, Olin E.] Purdue Univ, Dept Forestry & Nat Resources, W Lafayette, IN 47907 USA. RP Beasley, JC (reprint author), Univ Georgia, Savannah River Ecol Lab, Aiken, SC 29802 USA. EM beasley@srel.edu FU Department of Forestry; Natural Resources at Purdue University FX This study would not have been possible without the cooperation of numerous landowners who permitted us access to their land. We thank Z. Olson, G. Dharmarajan, W. Beatty, and T. Eagan for their assistance in the collection of field data. We also thank W. Clark and 1 anonymous reviewer for their numerous comments that improved this manuscript. Funding for this research was provided by the Department of Forestry and Natural Resources at Purdue University. NR 36 TC 7 Z9 7 U1 1 U2 45 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0022-541X EI 1937-2817 J9 J WILDLIFE MANAGE JI J. Wildl. Manage. PD NOV PY 2012 VL 76 IS 8 BP 1718 EP 1724 DI 10.1002/jwmg.423 PG 7 WC Ecology; Zoology SC Environmental Sciences & Ecology; Zoology GA 026DB UT WOS:000310252300022 ER PT J AU Ai, Y Marrone, BL AF Ai, Ye Marrone, Babetta L. TI Droplet translocation by focused surface acoustic waves SO MICROFLUIDICS AND NANOFLUIDICS LA English DT Article DE Microfluidics; Surface acoustic wave (SAW); Interdigital transducer (IDT); Acoustic streaming; Droplet manipulation ID BIOLOGICAL APPLICATIONS; MICROFLUIDICS; ACTUATION; VIEW AB This paper presents the experimental investigations of droplet movement driven by focused surface acoustic waves (SAWs) generated by a circular-arc interdigital transducer (CIDT). Surface acoustic waves propagating through a droplet in contact with the substrate exerted an acoustic streaming force on the droplet, as demonstrated by numerical modeling in this study. Different from the straight droplet movement driven by a straight interdigital transducer (SIDT), the droplets were focused to the center region of the CIDT. In addition, the droplets driven by the CIDT moved much faster than those driven by the SIDT with an identical input power because of the concentrated acoustic energy in the CIDT. Merging of two moving droplets using the CIDT was also demonstrated. The present results show that focused SAWs can be more efficient than uniform SAWs for droplet and fluid actuation in microfluidics. C1 [Ai, Ye; Marrone, Babetta L.] Los Alamos Natl Lab, Biosci Div, Los Alamos, NM 87545 USA. RP Marrone, BL (reprint author), Los Alamos Natl Lab, Biosci Div, POB 1663, Los Alamos, NM 87545 USA. EM blm@lanl.gov RI Ai, Ye/F-3411-2011 OI Ai, Ye/0000-0001-8638-1649 FU National Center for Research Resources; National Institute of General Medical Sciences of the National Institutes of Health [P41 RR01315]; National Flow Cytometry Resource; National Nuclear Security Administration of the US Department of Energy [DE-AC52-06NA25396] FX This work was supported from the National Center for Research Resources and the National Institute of General Medical Sciences of the National Institutes of Health through Grant Number P41 RR01315, the National Flow Cytometry Resource. This work was performed, in part, at the Center for Integrated Nanotechnologies, a US Department of Energy, Office of Basic Energy Sciences user facility and the authors gratefully acknowledge Mr. Jon Kevin Baldwin for the assistance of Cr/Au deposition. Los Alamos National Laboratory, an affirmative action equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the US Department of Energy under contract DE-AC52-06NA25396. NR 28 TC 20 Z9 20 U1 4 U2 42 PU SPRINGER HEIDELBERG PI HEIDELBERG PA TIERGARTENSTRASSE 17, D-69121 HEIDELBERG, GERMANY SN 1613-4982 J9 MICROFLUID NANOFLUID JI Microfluid. Nanofluid. PD NOV PY 2012 VL 13 IS 5 BP 715 EP 722 DI 10.1007/s10404-012-0990-y PG 8 WC Nanoscience & Nanotechnology; Instruments & Instrumentation; Physics, Fluids & Plasmas SC Science & Technology - Other Topics; Instruments & Instrumentation; Physics GA 031LG UT WOS:000310640900003 ER PT J AU Maguire, K Sullivan, M Ellis, RS Nugent, PE Howell, DA Gal-Yam, A Cooke, J Mazzali, P Pan, YC Dilday, B Thomas, RC Arcavi, I Ben-Ami, S Bersier, D Bianco, FB Fulton, BJ Hook, I Horesh, A Hsiao, E James, PA Podsiadlowski, P Walker, ES Yaron, O Kasliwal, MM Laher, RR Law, NM Ofek, EO Poznanski, D Surace, J AF Maguire, K. Sullivan, M. Ellis, R. S. Nugent, P. E. Howell, D. A. Gal-Yam, A. Cooke, J. Mazzali, P. Pan, Y-C Dilday, B. Thomas, R. C. Arcavi, I. Ben-Ami, S. Bersier, D. Bianco, F. B. Fulton, B. J. Hook, I. Horesh, A. Hsiao, E. James, P. A. Podsiadlowski, P. Walker, E. S. Yaron, O. Kasliwal, M. M. Laher, R. R. Law, N. M. Ofek, E. O. Poznanski, D. Surace, J. TI Hubble Space Telescope studies of low-redshift Type Ia supernovae: evolution with redshift and ultraviolet spectral trends SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Review DE supernovae: general; galaxies: general; distance scale; cosmological parameters ID DIGITAL SKY SURVEY; 2-PARAMETER LUMINOSITY CORRECTION; MASS-METALLICITY RELATION; HOST GALAXIES; LEGACY SURVEY; LIGHT CURVES; MAXIMUM BRIGHTNESS; LOW-RESOLUTION; STAR-FORMATION; WHITE-DWARF AB We present an analysis of the maximum light, near-ultraviolet (NUV; 2900 < lambda < 5500 angstrom) spectra of 32 low-redshift (0.001 < z < 0.08) Type Ia supernovae (SNe Ia), obtained with the Hubble Space Telescope (HST) using the Space Telescope Imaging Spectrograph. We combine this spectroscopic sample with high-quality gri light curves obtained with robotic telescopes to measure SN Ia photometric parameters, such as stretch (light-curve width), optical colour and brightness (Hubble residual). By comparing our new data to a comparable sample of SNe Ia at intermediate redshift (0.4 < z < 0.9), we detect modest spectral evolution (3s), in the sense that our mean low-redshift NUV spectrum has a depressed flux compared to its intermediate-redshift counterpart. We also see a strongly increased dispersion about the mean with decreasing wavelength, confirming the results of earlier surveys. We show that these trends are consistent with changes in metallicity as predicted by contemporary SN Ia spectral models. We also examine the properties of various NUV spectral diagnostics in the individual SN spectra. We find a general correlation between SN stretch and the velocity (or position) of many NUV spectral features. In particular, we observe that higher stretch SNe have larger Ca ii H&K velocities, which also correlate with host galaxy stellar mass. This latter trend is probably driven by the well-established correlation between stretch and host galaxy stellar mass. We find no significant trends between UV spectral features and optical colour. Mean spectra constructed according to whether the SN has a positive or negative Hubble residual show very little difference at NUV wavelengths, indicating that the NUV evolution and variation we identify does not directly correlate with Hubble diagram residuals. Our work confirms and strengthens earlier conclusions regarding the complex behaviour of SNe Ia in the NUV spectral region, but suggests the correlations we find are more useful in constraining progenitor models rather than improving the use of SNe Ia as cosmological probes. C1 [Maguire, K.; Sullivan, M.; Pan, Y-C; Hook, I.; Podsiadlowski, P.] Univ Oxford, Dept Phys Astrophys, DWB, Oxford OX1 3RH, England. [Ellis, R. S.; Horesh, A.; Surace, J.] CALTECH, Cahill Ctr Astrophys, Pasadena, CA 91125 USA. [Nugent, P. E.; Thomas, R. C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Cosmol Ctr, Berkeley, CA 94720 USA. [Nugent, P. E.] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. [Howell, D. A.; Dilday, B.; Bianco, F. B.; Fulton, B. J.] Las Cumbres Observ Global Telescope Network, Goleta, CA 93117 USA. [Howell, D. A.; Dilday, B.; Bianco, F. B.] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA. [Gal-Yam, A.; Arcavi, I.; Ben-Ami, S.; Yaron, O.; Ofek, E. O.] Weizmann Inst Sci, Astrophys Grp, IL-76100 Rehovot, Israel. [Cooke, J.] Swinburne Univ Technol, Hawthorn, Vic 3122, Australia. [Mazzali, P.] INAF Osservatorio Astron, I-35122 Padua, Italy. [Mazzali, P.] Max Planck Inst Astrophys, D-85748 Garching, Germany. [Bersier, D.; James, P. A.] Liverpool John Moores Univ, Astrophys Res Inst, Birkenhead CH41 1LD, Merseyside, England. [Hook, I.] INAF Osservatorio Astron Roma, I-00040 Rome, Italy. [Hsiao, E.] Las Campanas Observ, Carnegie Observ, La Serena, Chile. [Walker, E. S.] Scuola Normale Super Pisa, I-56126 Pisa, Italy. [Kasliwal, M. M.] Observ Carnegie Inst Sci, Pasadena, CA 91101 USA. [Laher, R. R.] CALTECH, Spitzer Sci Ctr, Pasadena, CA 91125 USA. [Law, N. M.] Univ Toronto, Dunlap Inst Astron & Astrophys, Toronto, ON M5S 3H4, Canada. [Poznanski, D.] Tel Aviv Univ, Sch Phys & Astron, IL-69978 Tel Aviv, Israel. RP Maguire, K (reprint author), Univ Oxford, Dept Phys Astrophys, DWB, Keble Rd, Oxford OX1 3RH, England. EM kate.maguire@astro.ox.ac.uk RI Horesh, Assaf/O-9873-2016; OI Horesh, Assaf/0000-0002-5936-1156; Sullivan, Mark/0000-0001-9053-4820; James, Philip/0000-0003-4131-5183 FU Royal Society; Weizmann-UK; ISF; BSF; Minerva grant; ARCHES award; Lord Sieff of Brompton Fund; Las Cumbres Observatory Global Telescope Network; Israeli Ministry of Science; NASA [NAS 5-26555]; UK Science and Technology Facilities Council; W. M. Keck Foundation; National Aeronautics and Space Administration; Hubble Fellowship; Carnegie-Princeton Fellowship FX MS acknowledges support from the Royal Society. AG-Y and MS acknowledge support from the Weizmann-UK 'making connections' programme. AG-Y further acknowledges support by the ISF, BSF, a Minerva grant, the ARCHES award and the Lord Sieff of Brompton Fund. DAH and BD are supported by the Las Cumbres Observatory Global Telescope Network. MMK acknowledges generous support from the Hubble Fellowship and Carnegie-Princeton Fellowship. EOO is incumbent of the Arye Dissentshik career development chair and is grateful to support by a grant from the Israeli Ministry of Science.; This paper is based on observations made with the NASA/ESA HST, obtained at the Space Telescope Science Institute, which is operated by the Association of Universities for Research in Astronomy, Inc., under NASA contract NAS 5-26555. These observations are associated with programmes 11721 and 12298. The Liverpool Telescope is operated on the island of La Palma by Liverpool John Moores University in the Spanish Observatorio del Roque de los Muchachos of the Instituto de Astrofisica de Canarias with financial support from the UK Science and Technology Facilities Council. Observations were obtained with the Samuel Oschin Telescope at the Palomar Observatory as part of the Palomar Transient Factory project, a scientific collaboration between the California Institute of Technology, Columbia University, La Cumbres Observatory, the Lawrence Berkeley National Laboratory, the National Energy Research Scientific Computing Center, the University of Oxford and the Weizmann Institute of Science. The William Herschel Telescope is operated on the island of La Palma by the Isaac Newton Group in the Spanish Observatorio del Roque de los Muchachos of the Instituto de Astrofisica de Canarias. Some of the data were obtained with the W. M. Keck Observatory, which is operated as a scientific partnership among the California Institute of Technology, the University of California and the National Aeronautics and Space Administration. These observations were made possible by the generous financial support of the W. M. Keck Foundation. This paper uses observations obtained with facilities of the LCOGT. The BOS is operated by the Las Cumbres Observatory Global Telescope Network and is located at the Sedgwick Reserve, a part of the University of California Natural Reserve System. This research has made use of the NASA/IPAC Extragalactic Database (NED) which is operated by the Jet Propulsion Laboratory, California Institute of Technology, under contract with the National Aeronautics and Space Administration. NR 104 TC 55 Z9 55 U1 0 U2 9 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD NOV PY 2012 VL 426 IS 3 BP 2359 EP 2379 DI 10.1111/j.1365-2966.2012.21909.x PG 21 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 023VE UT WOS:000310063900049 ER PT J AU Hafen, RP Henry, MJ AF Hafen, Ryan P. Henry, Michael J. TI Speech information retrieval: a review SO MULTIMEDIA SYSTEMS LA English DT Article DE Speech signal processing; Speech event detection; Speech classification; Speech segmentation; Speech analysis features; Speech recognition; Speaker recognition; Indexing and retrieval; Multilingual analysis; Acoustic fingerprinting ID INDEPENDENT SPEAKER VERIFICATION; LANGUAGE IDENTIFICATION; BROADCAST NEWS; AUDIO DATA; RECOGNITION; DIARIZATION; CLASSIFICATION; SEGMENTATION AB Speech is an information-rich component of multimedia. Information can be extracted from a speech signal in a number of different ways, and thus there are several well-established speech signal analysis research fields. These fields include speech recognition, speaker recognition, event detection, and fingerprinting. The information that can be extracted from tools and methods developed in these fields can greatly enhance multimedia systems. In this paper, we present the current state of research in each of the major speech analysis fields. The goal is to introduce enough background for someone new in the field to quickly gain high-level understanding and to provide direction for further study. C1 [Hafen, Ryan P.; Henry, Michael J.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Hafen, RP (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM ryan.hafen@pnnl.gov; michael.j.henry@pnnl.gov FU US Department of Energy [DE-AC05-76RL01830] FX This work has been supported by a government client. The Pacific Northwest National Laboratory is managed for the US Department of Energy by Battelle Memorial Institute under Contract DE-AC05-76RL01830. NR 128 TC 0 Z9 0 U1 1 U2 24 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0942-4962 EI 1432-1882 J9 MULTIMEDIA SYST JI Multimedia Syst. PD NOV PY 2012 VL 18 IS 6 BP 499 EP 518 DI 10.1007/s00530-012-0266-0 PG 20 WC Computer Science, Information Systems; Computer Science, Theory & Methods SC Computer Science GA 027AC UT WOS:000310323200004 ER PT J AU Arslan, I Stach, EA AF Arslan, Ilke Stach, Eric A. TI ELECTRON TOMOGRAPHY Seeing atoms in three dimensions SO NATURE MATERIALS LA English DT News Item C1 [Arslan, Ilke] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA USA. [Stach, Eric A.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Arslan, I (reprint author), Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA USA. EM Ilke.Arslan@pnnl.gov; EStach@BNL.gov RI Stach, Eric/D-8545-2011 OI Stach, Eric/0000-0002-3366-2153 NR 8 TC 4 Z9 4 U1 3 U2 57 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1476-1122 J9 NAT MATER JI Nat. Mater. PD NOV PY 2012 VL 11 IS 11 BP 911 EP 912 PG 2 WC Chemistry, Physical; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Materials Science; Physics GA 028PN UT WOS:000310434600008 PM 23089992 ER PT J AU Reichhardt, C Reichhardt, CO AF Reichhardt, Charles Reichhardt, Cynthia Olson TI DEFECT DYNAMICS Breaking up in a curved plane SO NATURE MATERIALS LA English DT News Item ID SPHERICAL CRYSTALLOGRAPHY C1 [Reichhardt, Charles; Reichhardt, Cynthia Olson] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Reichhardt, C (reprint author), Los Alamos Natl Lab, Div Theoret, POB 1663, Los Alamos, NM 87545 USA. EM reichhardt@lanl.gov NR 8 TC 0 Z9 0 U1 1 U2 10 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1476-1122 J9 NAT MATER JI Nat. Mater. PD NOV PY 2012 VL 11 IS 11 BP 912 EP 913 PG 3 WC Chemistry, Physical; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Materials Science; Physics GA 028PN UT WOS:000310434600009 PM 23089993 ER PT J AU Lee, SH Choi, M Kim, TT Lee, S Liu, M Yin, X Choi, HK Lee, SS Choi, CG Choi, SY Zhang, X Min, B AF Lee, Seung Hoon Choi, Muhan Kim, Teun-Teun Lee, Seungwoo Liu, Ming Yin, Xiaobo Choi, Hong Kyw Lee, Seung S. Choi, Choon-Gi Choi, Sung-Yool Zhang, Xiang Min, Bumki TI Switching terahertz waves with gate-controlled active graphene metamaterials SO NATURE MATERIALS LA English DT Article ID TRANSISTORS; MODULATOR; PLASMONICS; TRANSPORT; DEVICES; FILMS AB The extraordinary electronic properties of graphene provided the main thrusts for the rapid advance of graphene electronics(1). In photonics, the gate-controllable electronic properties of graphene provide a route to efficiently manipulate the interaction of photons with graphene, which has recently sparked keen interest in graphene plasmonics(2-10). However, the electro-optic tuning capability of unpatterned graphene alone is still not strong enough for practical optoelectronic applications owing to its non-resonant Drude-like behaviour. Here, we demonstrate that substantial gate-induced persistent switching and linear modulation of terahertz waves can be achieved in a two-dimensional metamaterial(11,12), into which an atomically thin, gated two-dimensional graphene layer is integrated. The gate-controllable light-matter interaction in the graphene layer can be greatly enhanced by the strong resonances of the metamaterial(13). Although the thickness of the embedded single-layer graphene is more than six orders of magnitude smaller than the wavelength ( infinity limit of a rate equation for a neutron population generating function, related to a rate equation studied by Feynman. The Bohnel equation is also shown to be a fixed point of an iteration problem, related to one studied by Hawkins and Ulam, where the iteration generates the chain a generation at a time. The discrete iteration problem is shown to be connected to the continuous time evolution of the chain. An explicit solution for the time evolution of the chain is given in the simplified approximation where at most two neutrons are created by an induced fission. The t -> infinity limit of this equation gives a simple analytic expression for the solution to the Bohnel equation in this approximation. A generalized Poisson counting distribution constructed from the theoretical fission chain probability number distribution is compared to experimental data for a multiplying Pu sample. C1 [Prasad, Manoj K.] Lawrence Livermore Natl Lab, WCI AX Div, Livermore, CA 94550 USA. [Snyderman, Neal J.] Lawrence Livermore Natl Lab, GS N Program, Livermore, CA 94550 USA. RP Prasad, MK (reprint author), Lawrence Livermore Natl Lab, WCI AX Div, POB 808,L-039, Livermore, CA 94550 USA. EM prasad1@llnl.gov FU U.S. Department of Energy by the Lawrence Livermore National Laboratory [W-7405-ENG-48] FX We would like to thank M. Rowland for stimulating our interest in this problem. We would also like to thank L. Nakae and P. Kerr for supplying us with the experimental data. We would also like to thank R. Cullen for discussions relating to generalized Poisson distributions. This work was performed under the auspices of the U.S. Department of Energy by the Lawrence Livermore National Laboratory under contract W-7405-ENG-48. NR 21 TC 10 Z9 10 U1 0 U2 5 PU AMER NUCLEAR SOC PI LA GRANGE PK PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA SN 0029-5639 EI 1943-748X J9 NUCL SCI ENG JI Nucl. Sci. Eng. PD NOV PY 2012 VL 172 IS 3 BP 300 EP 326 PG 27 WC Nuclear Science & Technology SC Nuclear Science & Technology GA 028AW UT WOS:000310396200007 ER PT J AU Sorensen, P AF Sorensen, Peter TI Importance of upgraded energy reconstruction for direct dark matter searches with liquid xenon detectors SO PHYSICAL REVIEW D LA English DT Article AB The usual nuclear recoil energy reconstruction employed by liquid xenon dark matter search experiments relies only on the primary scintillation photon signal. Energy reconstruction based on both the photon and electron signals yields a more accurate representation of search results. For a dark matter particle of mass m(chi) similar to 10 GeV, a nuclear recoil from a scattering event is more likely to be observed in the lower-left corner of the typical search box, rather than near the nuclear recoil calibration centroid. In this region of the search box, the actual nuclear recoil energies are smaller than the usual energy scale suggests, by about a factor of 2. Recent search results from the XENON100 experiment are discussed in light of these considerations. C1 Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Sorensen, P (reprint author), Lawrence Livermore Natl Lab, 7000 E Ave, Livermore, CA 94550 USA. EM pfs@llnl.gov FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX Thanks are due to Adam Bernstein, Rouven Essig, Rick Gaitskell, Jeremy Mardon, Neal Weiner and the XENON100 Collaboration, for suggesting improvements to the manuscript. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. Its report number is LLNL-TR-574054. NR 20 TC 6 Z9 6 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 1550-7998 J9 PHYS REV D JI Phys. Rev. D PD NOV 1 PY 2012 VL 86 IS 10 AR 101301 DI 10.1103/PhysRevD.86.101301 PG 4 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA 029MU UT WOS:000310500700001 ER PT J AU Durkee, JW AF Durkee, Joe W., Jr. TI MCNP geometry transformation and plotter equations SO PROGRESS IN NUCLEAR ENERGY LA English DT Article DE MCNP; MCNPX; Geometry; Transformation; Plot AB The MCNP Monte Carlo radiation-transport code contains versatile capabilities to develop and plot geometries used in simulations. Although these capabilities have been available in MCNP since the late 1970s, many of the derivational details underpinning these capabilities are not contained in the MCNP manual and do not appear to have been documented in Los Alamos reports or the published literature. Derivations of many of the equations underlying the MCNP geometry transformation and geometry plot utility are presented here. Although this document does not include derivations of all of the expressions contained in MCNP, its contents should nevertheless provide the reader with a deeper understanding of the geometry transformation and plotting features than can be obtained using only the MCNP theory manual. Published by Elsevier Ltd. C1 Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Durkee, JW (reprint author), Los Alamos Natl Lab, POB 1663,MS K575, Los Alamos, NM 87545 USA. EM jdurkee@lanl.gov NR 17 TC 1 Z9 1 U1 2 U2 5 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0149-1970 J9 PROG NUCL ENERG JI Prog. Nucl. Energy PD NOV PY 2012 VL 61 BP 26 EP 40 DI 10.1016/j.pnucene.2012.06.004 PG 15 WC Nuclear Science & Technology SC Nuclear Science & Technology GA 023NE UT WOS:000310040900003 ER PT J AU Jang, DH Anderson-Cook, CM Kim, Y AF Jang, Dae-Heung Anderson-Cook, Christine M. Kim, Youngil TI Three-Dimensional Quantile Plots and Dynamic Quantile Plots of the Prediction Variance for Response Surface Designs SO QUALITY AND RELIABILITY ENGINEERING INTERNATIONAL LA English DT Article DE graphical design assessment; second-order models; fraction of design space plots; variance dispersion graphs; quantile plots; dynamic quantile plots ID COMPARING DESIGNS; DISPERSION GRAPHS; CAPABILITY AB A historically common choice for evaluating response surface designs is to use alphabetic optimality criteria. Single-number criteria such as D, A, G, and V optimality do not completely reflect the estimation or prediction variance characteristics of the designs in question. For prediction-based assessment, alternatives to single-number summaries include the graphical displays of the prediction variance across the design regions. Variance dispersion graphs, fraction of design space plots, and quantile plots have been suggested to evaluate the overall prediction capability of response surface designs. The quantile plots use the percentiles. These quantile plots use the percentiles of the distribution at a given radius instead of just the mean, maximum, and minimum prediction variance values on concentric spheres inside the region of the interest. Previously, the user had to select several values of radius and draw corresponding quantile plots to evaluate the overall prediction capability of response surface designs. The user-specified choice of radii to examine makes the plot somewhat subjective. Alternately, we propose to remove this subjectivity by using a three-dimensional quantile plot. As another extension of the quantile plots, we suggest dynamic quantile plots to animate the quantile plots and use them for comparing and evaluating response surface designs. Copyright (C) 2011 John Wiley & Sons, Ltd. C1 [Jang, Dae-Heung] Pukyong Natl Univ, Dept Stat, Pusan, South Korea. [Anderson-Cook, Christine M.] Los Alamos Natl Lab, Stat Sci Grp, Los Alamos, NM USA. [Kim, Youngil] Chung Ang Univ, Dept Informat Syst, Seoul 156756, South Korea. RP Jang, DH (reprint author), Pukyong Natl Univ, Dept Stat, Pusan, South Korea. EM dhjang@pknu.ac.kr FU Basic Science Research Program through the National Research Foundation of Korea (NRF); Ministry of Education, Science and Technology [2010-0010794] FX This research was supported by the Basic Science Research Program through the National Research Foundation of Korea (NRF) funded by the Ministry of Education, Science and Technology (2010-0010794). NR 10 TC 0 Z9 0 U1 0 U2 2 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0748-8017 J9 QUAL RELIAB ENG INT JI Qual. Reliab. Eng. Int. PD NOV PY 2012 VL 28 IS 7 BP 713 EP 723 DI 10.1002/qre.1263 PG 11 WC Engineering, Multidisciplinary; Engineering, Industrial; Operations Research & Management Science SC Engineering; Operations Research & Management Science GA 029HX UT WOS:000310486600005 ER PT J AU Pintar, A Anderson-Cook, CM Wu, HQ AF Pintar, Adam Anderson-Cook, Christine M. Wu, Huaiqing TI Model Selection for Good Estimation and Prediction over a User-Specified Covariate Distribution for Linear Models under the Frequentist Paradigm SO QUALITY AND RELIABILITY ENGINEERING INTERNATIONAL LA English DT Article DE Akaike information criterion; correlated variables; cross validation; fraction of design space; mean squared error ID RESPONSE-SURFACE DESIGNS; VARIABLE SELECTION; CROSS-VALIDATION; FRACTION; SPACE AB Model selection is an important part of estimation and prediction for linear models with multiple explanatory variables (covariates). A variety of approaches exist that focus on the estimation of model parameters or the fit of the model where data have been observed. This article proposes an alternative strategy that selects models based on the mean squared error of the estimated expected response for a user-specified distribution of interest on the covariate space. We discuss numerical and graphical tools for detailed comparisons among different models. These tools help select a best model based on its ability to estimate the mean response over covariate locations likely to arise from a distribution of interest and can be combined with cost for deciding whether to include specific covariates. The proposed method is illustrated with three examples. We also present simulation results demonstrating situations where the proposed method shows improvement over some standard alternatives. Copyright (C) 2011 John Wiley & Sons, Ltd. C1 [Anderson-Cook, Christine M.] Los Alamos Natl Lab, Stat Sci Grp, Los Alamos, NM 87545 USA. [Pintar, Adam] NIST, Stat Engn Div, Gaithersburg, MD 20899 USA. [Wu, Huaiqing] Iowa State Univ, Dept Stat, Ames, IA 50011 USA. RP Anderson-Cook, CM (reprint author), Los Alamos Natl Lab, Stat Sci Grp, POB 1663, Los Alamos, NM 87545 USA. EM c-and-cook@lanl.gov NR 22 TC 1 Z9 1 U1 0 U2 5 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0748-8017 J9 QUAL RELIAB ENG INT JI Qual. Reliab. Eng. Int. PD NOV PY 2012 VL 28 IS 7 BP 767 EP 782 DI 10.1002/qre.1273 PG 16 WC Engineering, Multidisciplinary; Engineering, Industrial; Operations Research & Management Science SC Engineering; Operations Research & Management Science GA 029HX UT WOS:000310486600010 ER PT J AU Shagina, NB Vorobiova, MI Degteva, MO Peremyslova, LM Shishkina, EA Anspaugh, LR Napier, BA AF Shagina, N. B. Vorobiova, M. I. Degteva, M. O. Peremyslova, L. M. Shishkina, E. A. Anspaugh, L. R. Napier, B. A. TI Reconstruction of the contamination of the Techa River in 1949-1951 as a result of releases from the "MAYAK" Production Association SO RADIATION AND ENVIRONMENTAL BIOPHYSICS LA English DT Article DE Techa River; Liquid radioactive wastes; Radionuclide transport; Modeling ID DOSE ASSESSMENT; POPULATION AB More accurate reconstruction of the radioactive contamination of the Techa River system in 1949-1951 has been made on the basis of refined data on the amounts and the rate of discharge of radionuclides into the Techa River from the Mayak Production Association; this has led to the development of a modified Techa River model that describes the transport of radionuclides through the up-river ponds and along the Techa River and deposition of radionuclides in the river-bottom sediments and flooded areas. The refined Techa River source-term data define more precisely the time-dependent rates of release and radionuclide composition of the releases that occurred during 1949-1951. The Techa River model takes into account the time-dependent characteristics of the releases and considers (a) the transport of radionuclides adsorbed on solid particles originally contained in the discharges or originating in the up-river ponds as a result of stirring up of contaminated bottom sediments and (b) the transport of radionuclides in soluble form. The output of the Techa River model provides concentrations of all source-term radionuclides in the river water, bottom sediments, and floodplain soils at different distances from the site of radioactive releases for the period of major contamination in 1950-1951. The outputs of the model show good agreement with historical measurements of water and sediment contamination. In addition, the river-model output for Sr-90 concentration in the river water is harmonized with retrospective estimates derived from the measurements of Sr-90 in the residents of the Techa Riverside villages. Modeled contamination of the floodplain soils by Cs-137 is shown to be in agreement with the values reconstructed from late measurements of this radionuclide. Reconstructed estimates of the Techa River contamination are being used for the quantification of internal and external doses received by residents of the Techa Riverside communities. C1 [Shagina, N. B.; Vorobiova, M. I.; Degteva, M. O.; Peremyslova, L. M.; Shishkina, E. A.] Urals Res Ctr Radiat Med, Chelyabinsk 454076, Russia. [Anspaugh, L. R.] Univ Utah, Salt Lake City, UT USA. [Napier, B. A.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Shagina, NB (reprint author), Urals Res Ctr Radiat Med, 68A Vorovsky St, Chelyabinsk 454076, Russia. EM nata@urcrm.ru RI Shishkina, Elena/G-4595-2016; OI Shishkina, Elena/0000-0003-4464-0889; Shishkina, Elena/0000-0002-3076-2108 FU US Department of Energy's Office of Domestic and International Health Studies; US Environmental Protection Agency's Office of Radiation and Indoor Air; Federal Medical-Biological Agency of the Russian Federation FX This work has been funded by the US Department of Energy's Office of Domestic and International Health Studies, the US Environmental Protection Agency's Office of Radiation and Indoor Air, and the Federal Medical-Biological Agency of the Russian Federation. NR 35 TC 12 Z9 12 U1 0 U2 11 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0301-634X J9 RADIAT ENVIRON BIOPH JI Radiat. Environ. Biophys. PD NOV PY 2012 VL 51 IS 4 BP 349 EP 366 DI 10.1007/s00411-012-0414-0 PG 18 WC Biology; Biophysics; Environmental Sciences; Radiology, Nuclear Medicine & Medical Imaging SC Life Sciences & Biomedicine - Other Topics; Biophysics; Environmental Sciences & Ecology; Radiology, Nuclear Medicine & Medical Imaging GA 025WO UT WOS:000310227800001 PM 22797860 ER PT J AU Kogan, VG Prozorov, R AF Kogan, V. G. Prozorov, R. TI Orbital upper critical field and its anisotropy of clean one- and two-band superconductors SO REPORTS ON PROGRESS IN PHYSICS LA English DT Review ID SINGLE-CRYSTALS; MGB2; TEMPERATURE; PARAMETERS; DEPENDENCE; EQUATIONS AB The Helfand-Werthamer (HW) scheme (Helfand and Werthamer 1966 Phys. Rev. 147 288; another part of this work published as a separate paper by Werthamer et al 1966 Phys. Rev. 147 295) of evaluating the orbital upper critical field is generalized to anisotropic superconductors in general, and to two-band clean materials, in particular. Our formal procedure differs from those in the literature; it reproduces not only the isotropic HW limit but also the results of calculations for the two-band superconducting MgB2 (Miranovic et al 2003 J. Phys. Soc. Japan 72 221, Dahm and Schopohl 2003 Phys. Rev. Lett. 91 017001) along with the existing data on H-c2(T) and its anisotropy gamma(T) = H-c2,H-ab(T)/H-c2,H-c(T) (a, c are the principal directions of a uniaxial crystal). Using rotational ellipsoids as model Fermi surfaces we apply the formalism developed to study gamma(T) for a few different anisotropies of the Fermi surface and of the order parameters. We find that even for a single band d-wave order parameter gamma(T) decreases on warming; however, relatively weakly. For order parameters of the form Delta(k(z)) = Delta(0)(1 + eta cos k(z)a) (Xu et al 2011 Nature Phys. 7 198), according to our simulations gamma(T) may either increase or decrease on warming even for a single band depending on the sign of eta. Hence, the common belief that the multi-band Fermi surface is responsible for the temperature variation of gamma is proven incorrect. For two s-wave gaps, gamma decreases on warming for all Fermi shapes examined. For two order parameters of the form Delta(k(z)) = Delta(0)(1 + eta cos k(z)a), presumably relevant for pnictides, we obtain gamma(T) increasing on warming provided both eta(1) and eta(2) are negative, whereas for eta > 0, gamma(T) decreases. We study the ratio of the two order parameters at H-c2(T) and find that the ratio of the small gap to the large one does not vanish at any temperature, even at H-c2(T), an indication that this does not happen at lower fields. C1 [Kogan, V. G.] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. RP Kogan, VG (reprint author), Iowa State Univ, Ames Lab, Ames, IA 50011 USA. EM kogan@ameslab.gov; prozorov@ameslab.gov RI Prozorov, Ruslan/A-2487-2008 OI Prozorov, Ruslan/0000-0002-8088-6096 FU Department of Energy - Basic Energy Sciences [DE-AC02-07CH11358] FX Some ideas described in this text were conceived in discussions with Predrag Miranovich while working on Hc2(T) of MgB2 in 2002; VK is grateful to Predrag for this experience. We thank Andrey Chubukov for turning our attention to order parameters of the form (104) and our Ames Lab colleagues John Clem, Andreas Kreyssig, Sergey Bud'ko, Makariy Tanatar and Paul Canfield for interest and critique. We are grateful to Erick Blomberg for reading the manuscript and useful remarks. Work at the Ames Laboratory is supported by the Department of Energy - Basic Energy Sciences under Contract No DE-AC02-07CH11358. NR 50 TC 28 Z9 28 U1 2 U2 38 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0034-4885 J9 REP PROG PHYS JI Rep. Prog. Phys. PD NOV PY 2012 VL 75 IS 11 AR 114502 DI 10.1088/0034-4885/75/11/114502 PG 17 WC Physics, Multidisciplinary SC Physics GA 028WC UT WOS:000310454300003 PM 23085886 ER PT J AU Bailie, C McFarland, JA Greenough, JA Ranjan, D AF Bailie, C. McFarland, J. A. Greenough, J. A. Ranjan, D. TI Effect of incident shock wave strength on the decay of Richtmyer-Meshkov instability-introduced perturbations in the refracted shock wave SO SHOCK WAVES LA English DT Article DE Richtmyer-Meshkov instability; Shock wave refraction; Shock wave perturbation; Shock tube ID INITIAL CONDITIONS; TAYLOR AB The effect of incident shock wave strength on the decay of interface introduced perturbations in the refracted shock wave was studied by performing 20 different simulations with varying incident shock wave Mach numbers (M similar to 1.1- 3.5). The analysis showed that the amplitude decay can be represented as a power law model shown in Eq.7, where A is the average amplitude of perturbations (cm), B is the base constant (cm(-)(E-1), S is the distance travelled by the refracted shockwave (cm), and E is the power constant. The proposed model fits the data well for low incident Mach numbers, while at higher mach numbers the presence of large and irregular late time oscillations of the perturbation amplitude makes it hard for the power law to fit as effectively. When the coefficients from the power law decay model are plotted versus Mach number, a distinct transition region can be seen. This region is likely to result from the transition of the post-shock heavy gas velocity from subsonic to supersonic range in the lab frame. This region separates the data into a high and low Mach number region. Correlations for the power law coefficients to the incident shock Mach number are reported for the high and low Mach number regions. It is shown that perturbations in the refracted shock wave persist even at late times for high incident Mach numbers. C1 [Bailie, C.; McFarland, J. A.; Ranjan, D.] Texas A&M Univ, Dept Mech Engn, College Stn, TX 77843 USA. [Greenough, J. A.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Ranjan, D (reprint author), Texas A&M Univ, Dept Mech Engn, 3123 TAMU, College Stn, TX 77843 USA. EM dranjan@tamu.edu RI Bailie, Colin/K-8142-2013; OI Bailie, Colin/0000-0001-9203-2656; Ranjan, Devesh/0000-0002-1231-9313 FU HEDP summer student program at LLNL; US Department of Energy, Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; DOE-NNSA [DE-FG52-09NA29462] FX The authors would like to acknowledge the support of HEDP summer student program at LLNL, and to thank the scientists and staff that made this work possible. Also, we would like to thank, in particular, Mr. Cyrus Harrison for his data processing help and advice. This work was performed under the auspices of the US Department of Energy, Lawrence Livermore National Laboratory, under Contract No. DE-AC52-07NA27344. D.R. would also like to acknowledge the support of DOE-NNSA Grant No. DE-FG52-09NA29462. NR 29 TC 5 Z9 5 U1 0 U2 22 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0938-1287 J9 SHOCK WAVES JI Shock Waves PD NOV PY 2012 VL 22 IS 6 BP 511 EP 519 DI 10.1007/s00193-012-0382-y PG 9 WC Mechanics SC Mechanics GA 027BN UT WOS:000310326900003 ER PT J AU Balakrishnan, K Kuhl, AL Bell, JB Beckner, VE AF Balakrishnan, K. Kuhl, A. L. Bell, J. B. Beckner, V. E. TI An empirical model for the ignition of explosively dispersed aluminum particle clouds SO SHOCK WAVES LA English DT Article DE Blast wave; Turbulent mixing; Ignition; Dissociation; Ionization ID HYPERBOLIC CONSERVATION-LAWS; CHEMICAL EXPLOSIONS; SHOCK-WAVES; BLAST WAVES; COMBUSTION; POWDERS; GAS AB An empirical model for the ignition of aluminum particle clouds is developed and applied to the study of particle ignition and combustion behavior resulting from explosive blast waves. This model incorporates both particle ignition time delay as well as cloud concentration effects on ignition. The total mass of aluminum that burns is found to depend on the model, with shorter ignition delay times resulting in increased burning of the cloud. After the Al particles ignite, a competition for oxidizer between the booster detonation products and Al ensues. A new mass-averaged ignition parameter is defined and is observed to serve as a useful parameter to compare cloud ignition behavior. Investigation of this variable reveals that both peak ignition as well as the time required to attain peak ignition, are sensitive to the model parameters. The peak degree of dissociation in the fireball is about 19 % and the associated energy can play a significant role on the dynamics of the problem. The peak degree of ionization is about 2.9 % and the energy associated with this is much lower than the other controlling factors. Overall, this study demonstrates that the new ignition model developed captures effects not included in other combustion models for the investigation of shock-induced ignition of aluminum particle clouds. C1 [Balakrishnan, K.; Bell, J. B.; Beckner, V. E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, Berkeley, CA 94720 USA. [Kuhl, A. L.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RP Balakrishnan, K (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM kaushikb@lbl.gov FU U.S. Department of Energy by the Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Defense Threat Reduction Agency; [DE-AC02-05CH11231] FX This research work was performed under the auspices of the U.S. Department of Energy by the Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344, and supported by the Defense Threat Reduction Agency. The work at Lawrence Berkeley National Laboratory was performed under contract number DE-AC02-05CH11231. The simulations were performed at the ERDC High Performance Computing Center. The first author acknowledges interesting discussions held with Prof. David Frost of McGill University and Dr. Christer Fureby of the Swedish Defence Research Agency. NR 36 TC 0 Z9 0 U1 3 U2 18 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0938-1287 J9 SHOCK WAVES JI Shock Waves PD NOV PY 2012 VL 22 IS 6 BP 591 EP 603 DI 10.1007/s00193-012-0388-5 PG 13 WC Mechanics SC Mechanics GA 027BN UT WOS:000310326900010 ER PT J AU Kityk, IV AlZayed, N Lakshminarayana, G Wojciechowski, A Plucinski, KJ AF Kityk, I. V. AlZayed, N. Lakshminarayana, G. Wojciechowski, A. Plucinski, K. J. TI Photoinduced spectra for magneto electric (1-x)BiFeO3-xCuFe2O4 nanocomposites SO SPECTROCHIMICA ACTA PART A-MOLECULAR AND BIOMOLECULAR SPECTROSCOPY LA English DT Article DE Spectral properties of solids; Magnetooptical spectra ID CRYSTALS; RAMAN AB In this work, we demonstrate possibility to use spectra of the parametrically tuned laser beam for operation by magnetoelectric properties of the (1 - x)BiFeO3-xCuFe2O4 (BFCl). The role of the photoexcited wavelength is crucial due to photoexcited phonons. It may indicate on a spectral sensitivity of the studied nanocomposites. We have studied spectral dependences of magneto-electric constant versus the magnetic field frequency for different sizes of the nanoparticles with and without the nanosecond laser pulses illumination and we have shown an occurrence of principal spectral shifts in the corresponding magnetoelectric maxima. Additionally we have explored relative changes of dielectric permittivity and coercivity versus different photoinducing wavelengths. The performed experiments unambiguously show that the external laser treatment will lead to substantial shift of corresponding dielectric and magnetic parameters in the studied nanocomposites. It is principally the finding of clear spectral dependences for the mentioned dielectric and magnetic parameters. One can see their sensitivity to the photoinduced wavelength which reflects the photoexcitations of different part of wavelengths. One can see the spectral shift up to 100 nm for the two principal spectral maxima with respect to the dielectric and magnetic changes which may indicate on the two principally different contributions to the effects observed. (C) 2012 Elsevier B.V. All rights reserved. C1 [Kityk, I. V.; Wojciechowski, A.] Czestochowa Tech Univ, Dept Elect Engn, Czestochowa, Poland. [Kityk, I. V.; AlZayed, N.] King Saud Univ, Coll Sci, Dept Phys & Astron, Riyadh 11451, Saudi Arabia. [Lakshminarayana, G.] Los Alamos Natl Lab, Mat Sci & Technol Div MST 7, Los Alamos, NM 87545 USA. [Plucinski, K. J.] Mil Univ Technol, Dept Elect, PL-00908 Warsaw, Poland. RP Kityk, IV (reprint author), Czestochowa Tech Univ, Dept Elect Engn, Armii Krajowej 17, Czestochowa, Poland. EM iwank74@gmail.com RI Kityk, Iwan/M-4032-2015; OI Gandham, Lakshminarayana/0000-0002-1458-9368 NR 9 TC 0 Z9 0 U1 0 U2 12 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1386-1425 J9 SPECTROCHIM ACTA A JI Spectroc. Acta Pt. A-Molec. Biomolec. Spectr. PD NOV PY 2012 VL 97 BP 695 EP 698 DI 10.1016/j.saa.2012.07.021 PG 4 WC Spectroscopy SC Spectroscopy GA 028AS UT WOS:000310395800091 PM 22885117 ER PT J AU Ebert-McNeill, A Clark, SP Miller, JJ Birdsall, P Chandar, M Wu, L Cerny, EA Hall, PH Johnson, MH Isales, C Chutkan, N Bhattacharyya, MH AF Ebert-McNeill, Andrea Clark, Sara P. Miller, James J. Birdsall, Paige Chandar, Manisha Wu, Lucia Cerny, Elizabeth A. Hall, Patricia H. Johnson, Maribeth H. Isales, Carlos Chutkan, Norman Bhattacharyya, Maryka H. TI Cadmium Intake and Systemic Exposure in Postmenopausal Women and Age-Matched Men Who Smoke Cigarettes SO TOXICOLOGICAL SCIENCES LA English DT Article DE cigarette smoking; inhaled cadmium; blood cadmium; sensitive sub-population ID ATOMIC-ABSORPTION SPECTROPHOTOMETRY; PLASMA-MASS SPECTROMETRY; URINARY CADMIUM; SUNFLOWER KERNELS; TOBACCO-SMOKE; IRON STATUS; BLOOD; METALS; LEAD; POPULATION AB Mean blood cadmium (B-Cd) concentrations are two- to threefold higher in smokers than in nonsmokers. The basis for this phenomenon is not well understood. We conducted a detailed, multifaceted study of cadmium exposure in smokers. Groups were older smokers (624 years, n 25, 20% male) and nonsmokers (623 years, n 16, 31% male). Each subject's cigarettes were machine smoked, generating individually paired measures of inhaled cadmium (I-Cd) versus B-Cd; I-Cd and B-Cd were each evaluated three times, at monthly intervals. Urine cadmium (U-Cd) was analyzed for comparison. In four smokers, a duplicate-diet study was conducted, along with a kinetic study of plasma cadmium versus B-Cd. Female smokers had a mean B-Cd of 1.21ng Cd/ml, with a nearly 10-fold range (0.292.74ng Cd/ml); nonsmokers had a lower mean B-Cd, 0.35ng Cd/ml (p < 0.05), and narrower range (0.200.61ng Cd/ml). Means and ranges for males were similar. Estimates of cadmium amounts inhaled daily for our subjects smoking epsilon 20 cigarettes/day were far less than the 15 g Cd reported to be ingested daily via diet. This I-Cd amount was too low to alone explain the 3.5-fold elevation of B-Cd in our smokers, even assuming greater cadmium absorption via lungs than gastrointestinal tract; cadmium accumulated in smokers' lungs may provide the added cadmium. Finally, B-Cd appeared to be linearly related to I-Cd values in 75% of smokers, whereas 25% had far higher B-Cd, implying a possible heterogeneity among smokers regarding circulating cadmium concentrations and potentially cadmium toxicity. C1 [Bhattacharyya, Maryka H.] Georgia Hlth Sci Univ, Med Coll Georgia, Augusta, GA 30912 USA. [Ebert-McNeill, Andrea; Clark, Sara P.; Miller, James J.; Birdsall, Paige; Chandar, Manisha; Wu, Lucia; Cerny, Elizabeth A.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Bhattacharyya, MH (reprint author), Georgia Hlth Sci Univ, Med Coll Georgia, 1467 Harper St,HB 5025, Augusta, GA 30912 USA. EM mbhattacharyya@georgiahealth.edu RI Isales, Carlos/J-9902-2013 OI Isales, Carlos/0000-0002-4480-3484 FU Philip Morris USA; Philip Morris International; Philip Morris USA, Inc; Department of Medicine, Medical College of Georgia, Georgia Health Sciences University; Department of Orthopaedic Surgery, Medical College of Georgia, Georgia Health Sciences University FX The research supported by Philip Morris USA and Philip Morris International was funded through an Extramural Research Program managed by the Research Management Group (Linthicum Heights, MD). Philip Morris had no influence on the research conducted or the content of this publication.; Philip Morris USA, Inc, and Philip Morris International; Departments of Medicine and Orthopaedic Surgery, Medical College of Georgia, Georgia Health Sciences University. NR 67 TC 14 Z9 14 U1 0 U2 7 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 1096-6080 J9 TOXICOL SCI JI Toxicol. Sci. PD NOV PY 2012 VL 130 IS 1 BP 191 EP 204 DI 10.1093/toxsci/kfs226 PG 14 WC Toxicology SC Toxicology GA 025CV UT WOS:000310163200017 PM 22831969 ER PT J AU Hu, HC Yang, C Zhao, K AF Hu, Hua-Chen Yang, Chao Zhao, Kai TI Absorption correction A* for cylindrical and spherical samples with extended range and high accuracy calculated by the Thorkildsen and Larsen analytical method SO ACTA CRYSTALLOGRAPHICA SECTION A LA English DT Article ID RAPID CALCULATION; CYLINDERS; SPHERES; DIFFRACTION; EXTINCTION; CRYSTALS AB Tables of the absorption correction A* for cylindrical and spherical crystals were calculated by the Thorkildsen & Larsen [Acta Cryst. (1998), A54, 186-190] analytical method in the range of 0 <= mu R <= 30 and 0 <= theta <= 90 degrees with accuracies of 10(-6) for cylindrical crystals and 2.0 x 10(-6) for spherical crystals. Bivariate Chebyshev polynomial fitting formulae for A* are also provided for both cases. The maximum fitting error for spherical crystals is 6 x 10(-3) and the average error ranges from 7 x 10(-5) to 3 x 10(-4). All the important tables and the fitting program are provided in the supplementary material. C1 [Hu, Hua-Chen; Zhao, Kai] China Inst Atom Energy, Beijing 102413, Peoples R China. [Yang, Chao] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Computat Res Div, Berkeley, CA 94720 USA. RP Hu, HC (reprint author), China Inst Atom Energy, POB 275 18, Beijing 102413, Peoples R China. EM hchu3310@gmail.com; cyang@lbl.gov NR 10 TC 0 Z9 0 U1 2 U2 8 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0108-7673 J9 ACTA CRYSTALLOGR A JI Acta Crystallogr. Sect. A PD NOV PY 2012 VL 68 BP 778 EP 779 DI 10.1107/S0108767312039505 PN 6 PG 2 WC Chemistry, Multidisciplinary; Crystallography SC Chemistry; Crystallography GA 023DR UT WOS:000310013600011 PM 23075619 ER PT J AU Baker, EN Dauter, Z AF Baker, Edward N. Dauter, Zbigniew TI Nobel Prize for Chemistry 2012: GPCRs seen through a crystal ball SO ACTA CRYSTALLOGRAPHICA SECTION D-BIOLOGICAL CRYSTALLOGRAPHY LA English DT Editorial Material ID RECEPTOR C1 [Baker, Edward N.] Univ Auckland, Sch Biol Sci, Auckland 1, New Zealand. [Dauter, Zbigniew] Argonne Natl Lab, Biosci Div, Argonne, IL 60439 USA. RP Baker, EN (reprint author), Univ Auckland, Sch Biol Sci, Private Bag 92-019, Auckland 1, New Zealand. NR 4 TC 0 Z9 0 U1 0 U2 2 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0907-4449 J9 ACTA CRYSTALLOGR D JI Acta Crystallogr. Sect. D-Biol. Crystallogr. PD NOV PY 2012 VL 68 BP 1439 EP 1440 DI 10.1107/S0907444912043107 PN 11 PG 2 WC Biochemical Research Methods; Biochemistry & Molecular Biology; Biophysics; Crystallography SC Biochemistry & Molecular Biology; Biophysics; Crystallography GA 023XA UT WOS:000310069500001 PM 23090392 ER PT J AU Broadley, SG Gumbart, JC Weber, BW Marakalala, MJ Steenkamp, DJ Sewell, BT AF Broadley, Simon Gareth Gumbart, James Conrad Weber, Brandon William Marakalala, Mohlopheni Jackson Steenkamp, Daniel Jacobus Sewell, Bryan Trevor TI A new crystal form of MshB from Mycobacterium tuberculosis with glycerol and acetate in the active site suggests the catalytic mechanism SO ACTA CRYSTALLOGRAPHICA SECTION D-BIOLOGICAL CRYSTALLOGRAPHY LA English DT Article ID MOLECULAR-DYNAMICS; DEACETYLASE MSHB; MYCOTHIOL; BIOSYNTHESIS; REFINEMENT; REVEALS; SYSTEM; FIELD AB MshB, a zinc-based deacetylase, catalyses a step in the mycothiol biosynthetic pathway that involves the deacetylation of 1-O-(2-acetamido-2-deoxy-alpha-D-glucopyranosyl)-D-myo-inositol (GlcNAc-Ins), via cleavage of an amide bond, to 1-O-(2-amino-2-deoxy-alpha-D-glucopyranosyl)-D-myo-inositol (GlcN-Ins) and acetate. In this study, MshB was expressed, purified and crystallized. A new crystal form was encountered in 0.1 M sodium acetate, 0.2 M ammonium sulfate, 25% PEG 4000 pH 4.6. The crystals diffracted to 1.95 angstrom resolution and the resulting electron-density map revealed glycerol and the reaction product, acetate, in the active site. These ligands enabled the natural substrate GlcNAc-Ins to be modelled in the active site with some certainty. One acetate O atom is hydrogen bonded to Tyr142 and is located 2.5 angstrom from the catalytic zinc. The other acetate O atom is located 2.7 angstrom from a carboxylate O atom of Asp15. This configuration strongly suggests that Asp15 acts both as a general base catalyst in the nucleophilic attack of water on the amide carbonyl C atom and in its protonated form acts as a general acid to protonate the amide N atom. The configuration of Tyr142 differs from that observed previously in crystal structures of MshB (PDB entries 1q74 and 1q7t) and its location provides direct structural support for recently published biochemical and mutational studies suggesting that this residue is involved in a conformational change on substrate binding and contributes to the oxyanion hole that stabilizes the tetrahedral intermediate. C1 [Weber, Brandon William; Marakalala, Mohlopheni Jackson; Steenkamp, Daniel Jacobus; Sewell, Bryan Trevor] Univ Cape Town, Dept Clin Lab Sci, ZA-7700 Observatory, Western Cape, South Africa. [Sewell, Bryan Trevor] Univ Cape Town, Inst Infect Dis & Mol Med, ZA-7700 Observatory, Western Cape, South Africa. [Gumbart, James Conrad] Argonne Natl Lab, Biosci Div, Argonne, IL 60439 USA. [Broadley, Simon Gareth] Univ Cape Town, Dept Mol & Cell Biol, ZA-7700 Rondebosch, Western Cape, South Africa. RP Sewell, BT (reprint author), Univ Cape Town, Dept Clin Lab Sci, ZA-7700 Observatory, Western Cape, South Africa. EM trevor.sewell@uct.ac.za OI Broadley, Simon/0000-0001-8292-8213; MARAKALALA, MOHLOPHENI /0000-0001-7476-1652 FU National Research Foundation (NRF); UCT Drug Discovery Signature Theme; Argonne National Laboratory; Canon Collins Trust; NRF FX We would like to thank Dr Hassan Belrhali of EMBL Grenoble for making beam time available on BM14. SGB would like to thank the National Research Foundation (NRF) and the UCT Drug Discovery Signature Theme for financial support. JCG is supported by a Director's Postdoctoral Fellowship from Argonne National Laboratory. MJM acknowledges funding from the Canon Collins Trust and NRF. We would like to thank Professor David Gammon for his encouragement and useful comments on the manuscript and Dr Andrew McCarthy for providing the structure factors for the MshB structure with PDB code 1q7t. We would like to thank the co-editor and the referees for their comments and suggestions. In particular, we thank Professor Mike James, who suggested that we include the mechanism diagrams and perform the molecular-dynamics simulation and contributed the insight concerning the movement of Asp95 on substrate binding. NR 27 TC 6 Z9 6 U1 0 U2 9 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0907-4449 J9 ACTA CRYSTALLOGR D JI Acta Crystallogr. Sect. D-Biol. Crystallogr. PD NOV PY 2012 VL 68 BP 1450 EP 1459 DI 10.1107/S090744491203449X PN 11 PG 10 WC Biochemical Research Methods; Biochemistry & Molecular Biology; Biophysics; Crystallography SC Biochemistry & Molecular Biology; Biophysics; Crystallography GA 023XA UT WOS:000310069500003 PM 23090394 ER PT J AU Chacko, AR Zwart, PH Read, RJ Dodson, EJ Rao, CD Suguna, K AF Chacko, Anita R. Zwart, Peter H. Read, Randy J. Dodson, Eleanor J. Rao, C. D. Suguna, Kaza TI Severe diffraction anisotropy, rotational pseudosymmetry and twinning complicate the refinement of a pentameric coiled-coil structure of NSP4 of rotavirus SO ACTA CRYSTALLOGRAPHICA SECTION D-BIOLOGICAL CRYSTALLOGRAPHY LA English DT Article ID ENTEROTOXIGENIC PROTEIN NSP4; NONSTRUCTURAL GLYCOPROTEIN; INTRACELLULAR CALCIUM; MOLECULAR REPLACEMENT; CRYSTAL-STRUCTURE; PSEUDO-SYMMETRY; INTERACTS; MEMBRANE; SOFTWARE; DOMAIN AB The crystal structure of the region spanning residues 95-146 of the rotavirus nonstructural protein NSP4 from the asymptomatic human strain ST3 was determined at a resolution of 2.5 angstrom. Severe diffraction anisotropy, rotational pseudo-symmetry and twinning complicated the refinement of this structure. A systematic explanation confirming the crystal pathologies and describing how the structure was successfully refined is given in this report. C1 [Chacko, Anita R.; Suguna, Kaza] Indian Inst Sci, Mol Biophys Unit, Bangalore 560012, Karnataka, India. [Zwart, Peter H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Read, Randy J.] Univ Cambridge, Dept Haematol, Cambridge Inst Med Res, Cambridge CB2 2XY, England. [Dodson, Eleanor J.] Univ York, Dept Chem, York Struct Biol Lab, York YO10 5YW, N Yorkshire, England. [Rao, C. D.] Indian Inst Sci, Dept Microbiol & Cell Biol, Bangalore 560012, Karnataka, India. RP Suguna, K (reprint author), Indian Inst Sci, Mol Biophys Unit, CV Raman Ave, Bangalore 560012, Karnataka, India. EM suguna@mbu.iisc.ernet.in RI Read, Randy/L-1418-2013 OI Read, Randy/0000-0001-8273-0047 FU Indian Council of Medical Research; Department of Biotechnology (DBT); University Grants Commission (UGC), Government of India FX This work was supported by the Indian Council of Medical Research and the Department of Biotechnology (DBT) Infrastructure Program to the Indian Institute of Science. Preliminary data were collected at the X-ray Facility for Structural Biology in the Molecular Biophysics Unit of the Institute funded by the DBT. We thank J. Jeyakanthan, K. Sekar and G. Ueno for synchrotron data collection and processing. ARC acknowledges the University Grants Commission (UGC), Government of India for the award of a fellowship. NR 51 TC 4 Z9 4 U1 0 U2 4 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0907-4449 J9 ACTA CRYSTALLOGR D JI Acta Crystallogr. Sect. D-Biol. Crystallogr. PD NOV PY 2012 VL 68 BP 1541 EP 1548 DI 10.1107/S090744491203836X PN 11 PG 8 WC Biochemical Research Methods; Biochemistry & Molecular Biology; Biophysics; Crystallography SC Biochemistry & Molecular Biology; Biophysics; Crystallography GA 023XA UT WOS:000310069500012 PM 23090403 ER PT J AU Sierra, RG Laksmono, H Kern, J Tran, R Hattne, J Alonso-Mori, R Lassalle-Kaiser, B Glockner, C Hellmich, J Schafer, DW Echols, N Gildea, RJ Grosse-Kunstleve, RW Sellberg, J McQueen, TA Fry, AR Messerschmidt, MM Miahnahri, A Seibert, MM Hampton, CY Starodub, D Loh, ND Sokaras, D Weng, TC Zwart, PH Glatzel, P Milathianaki, D White, WE Adams, PD Williams, GJ Boutet, S Zouni, A Messinger, J Sauter, NK Bergmann, U Yano, J Yachandra, VK Bogan, MJ AF Sierra, Raymond G. Laksmono, Hartawan Kern, Jan Rosalie Tran Hattne, Johan Alonso-Mori, Roberto Lassalle-Kaiser, Benedikt Gloeckner, Carina Hellmich, Julia Schafer, Donald W. Echols, Nathaniel Gildea, Richard J. Grosse-Kunstleve, Ralf W. Sellberg, Jonas McQueen, Trevor A. Fry, Alan R. Messerschmidt, Marc M. Miahnahri, Alan Seibert, M. Marvin Hampton, Christina Y. Starodub, Dmitri Loh, N. Duane Sokaras, Dimosthenis Weng, Tsu-Chien Zwart, Petrus H. Glatzel, Pieter Milathianaki, Despina White, William E. Adams, Paul D. Williams, Garth J. Boutet, Sebastien Zouni, Athina Messinger, Johannes Sauter, Nicholas K. Bergmann, Uwe Yano, Junko Yachandra, Vittal K. Bogan, Michael J. TI Nanoflow electrospinning serial femtosecond crystallography SO ACTA CRYSTALLOGRAPHICA SECTION D-BIOLOGICAL CRYSTALLOGRAPHY LA English DT Article ID PROTEIN-STRUCTURE DETERMINATION; PHOTOSYSTEM-II; NANOCRYSTALLOGRAPHY; DIFFRACTION; CRYSTALS AB An electrospun liquid microjet has been developed that delivers protein microcrystal suspensions at flow rates of 0.14-3.1 mu l min(-1) to perform serial femtosecond crystallography (SFX) studies with X-ray lasers. Thermolysin microcrystals flowed at 0.17 mu l min(-1) and diffracted to beyond 4 angstrom resolution, producing 14 000 indexable diffraction patterns, or four per second, from 140 mu g of protein. Nanoflow electrospinning extends SFX to biological samples that necessitate minimal sample consumption. C1 [Sierra, Raymond G.; Laksmono, Hartawan; Hampton, Christina Y.; Starodub, Dmitri; Loh, N. Duane; Bogan, Michael J.] SLAC Natl Accelerator Lab, PULSE Inst, Menlo Pk, CA 94025 USA. [Kern, Jan; Rosalie Tran; Hattne, Johan; Lassalle-Kaiser, Benedikt; Echols, Nathaniel; Gildea, Richard J.; Grosse-Kunstleve, Ralf W.; Zwart, Petrus H.; Adams, Paul D.; Sauter, Nicholas K.; Yano, Junko; Yachandra, Vittal K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Kern, Jan; Alonso-Mori, Roberto; Schafer, Donald W.; Fry, Alan R.; Messerschmidt, Marc M.; Miahnahri, Alan; Seibert, M. Marvin; Milathianaki, Despina; White, William E.; Williams, Garth J.; Boutet, Sebastien; Bergmann, Uwe] SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA 94025 USA. [Gloeckner, Carina; Hellmich, Julia; Zouni, Athina] Tech Univ Berlin, Max Volmer Lab Biophys Chem, D-10623 Berlin, Germany. [Sellberg, Jonas; Sokaras, Dimosthenis; Weng, Tsu-Chien] SLAC Natl Accelerator Lab, SSRL, Menlo Pk, CA 94025 USA. [Sellberg, Jonas] Stockholm Univ, Dept Phys, AlbaNova, S-10691 Stockholm, Sweden. [McQueen, Trevor A.] Stanford Univ, Dept Chem, Menlo Pk, CA 94025 USA. [Glatzel, Pieter] European Synchrotron Radiat Facil, F-38043 Grenoble, France. [Messinger, Johannes] Umea Univ, Inst Kemi, Kemiskt Biol Ctr, Umea, Sweden. RP Bogan, MJ (reprint author), SLAC Natl Accelerator Lab, PULSE Inst, Menlo Pk, CA 94025 USA. EM mbogan@slac.stanford.edu RI Messerschmidt, Marc/F-3796-2010; Sauter, Nicholas/K-3430-2012; Adams, Paul/A-1977-2013; Bogan, Mike/I-6962-2012; Kern, Jan/G-2586-2013; Glatzel, Pieter/E-9958-2010; Loh, Duane/I-7371-2013; Sellberg, Jonas/C-6506-2009; Sokaras, Dimosthenis/G-6037-2010; Gildea, Richard/J-6862-2012; alonso-mori, roberto/G-2638-2013 OI Messerschmidt, Marc/0000-0002-8641-3302; Adams, Paul/0000-0001-9333-8219; Bogan, Mike/0000-0001-9318-3333; Kern, Jan/0000-0002-7272-1603; Glatzel, Pieter/0000-0001-6532-8144; Loh, Duane/0000-0002-8886-510X; Sellberg, Jonas/0000-0003-2793-5052; Sokaras, Dimosthenis/0000-0001-8117-1933; Gildea, Richard/0000-0001-5038-6958; alonso-mori, roberto/0000-0002-5357-0934 FU AMOS program, Office of Science, Office of Basic Energy Sciences (OBES), Division of Chemical Sciences, Geosciences and Biosciences (CSGB) of the Department of Energy (DOE); LCLS; SLAC Laboratory Directed Research and Development Program; OBES, CSGB of the DOE [DE-AC02-05CH11231]; Office of Science, DOE [DE-AC02-05CH11231]; NIH [GM 55302]; DFG-Cluster of Excellence 'UniCat'; Solar Fuels Strong Research Environment (Umea University); Artificial Leaf Project (K&A Wallenberg Foundation); VR FX The nanoflow liquid microjet work was supported by the AMOS program, Office of Science, Office of Basic Energy Sciences (OBES), Division of Chemical Sciences, Geosciences and Biosciences (CSGB) of the Department of Energy (DOE) (MJB), LCLS (MJB and DWS) and through the SLAC Laboratory Directed Research and Development Program (MJB and HL). This work was also supported by OBES, CSGB of the DOE under Contract DE-AC02-05CH11231 (JY and VKY) for structural studies and instrumentation, Director, Office of Science, DOE under Contract DE-AC02-05CH11231 (NKS) for data-processing methods and NIH Grant GM 55302 (VKY) for PS II biochemistry. In addition, the DFG-Cluster of Excellence 'UniCat' coordinated by the Technische Universitat Berlin (AZ), the Solar Fuels Strong Research Environment (Umea University; JM), the Artificial Leaf Project (K&A Wallenberg Foundation; JM) and VR (JM) are acknowledged for supporting this project. Experiments were carried out at the LCLS at SLAC National Accelerator Laboratory operated by Stanford University on behalf of DOE, OBES. We thank the staff at LCLS/SLAC for their support. NR 22 TC 62 Z9 62 U1 1 U2 52 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0907-4449 J9 ACTA CRYSTALLOGR D JI Acta Crystallogr. Sect. D-Biol. Crystallogr. PD NOV PY 2012 VL 68 BP 1584 EP 1587 DI 10.1107/S0907444912038152 PN 11 PG 4 WC Biochemical Research Methods; Biochemistry & Molecular Biology; Biophysics; Crystallography SC Biochemistry & Molecular Biology; Biophysics; Crystallography GA 023XA UT WOS:000310069500017 PM 23090408 ER PT J AU Moeller, SJ Tomasi, D Woicik, PA Maloney, T Alia-Klein, N Honorio, J Telang, F Wang, GJ Wang, RL Sinha, R Carise, D Astone-Twerell, J Bolger, J Volkow, ND Goldstein, RZ AF Moeller, Scott J. Tomasi, Dardo Woicik, Patricia A. Maloney, Thomas Alia-Klein, Nelly Honorio, Jean Telang, Frank Wang, Gene-Jack Wang, Ruiliang Sinha, Rajita Carise, Deni Astone-Twerell, Janetta Bolger, Joy Volkow, Nora D. Goldstein, Rita Z. TI Enhanced midbrain response at 6-month follow-up in cocaine addiction, association with reduced drug-related choice SO ADDICTION BIOLOGY LA English DT Article DE Cocaine addiction; dopamine; drug Stroop; fMRI; midbrain; thalamus ID ANTERIOR CINGULATE CORTEX; SELF-ADMINISTER COCAINE; BRAIN ACTIVATION; METHAMPHETAMINE ABUSERS; DEPENDENT INDIVIDUALS; DOPAMINE TRANSPORTERS; PROTRACTED ABSTINENCE; COGNITIVE CONTROL; DECISION-MAKING; FRONTAL-CORTEX AB Drug addiction is characterized by dysregulated dopamine neurotransmission. Although dopamine functioning appears to partially recover with abstinence, the specific regions that recover and potential impact on drug seeking remain to be determined. Here we used functional magnetic resonance imaging (fMRI) to study an ecologically valid sample of 15 treatment-seeking cocaine addicted individuals at baseline and 6-month follow-up. At both study sessions, we collected fMRI scans during performance of a drug Stroop task, clinical self-report measures of addiction severity and behavioral measures of cocaine seeking (simulated cocaine choice); actual drug use in between the two study sessions was also monitored. At 6-month follow-up (compared with baseline), we predicted functional enhancement of dopaminergically innervated brain regions, relevant to the behavioral responsiveness toward salient stimuli. Consistent with predictions, whole-brain analyses revealed responses in the midbrain (encompassing the ventral tegmental area/substantia nigra complex) and thalamus (encompassing the mediodorsal nucleus) that were higher (and more positively correlated) at follow-up than baseline. Increased midbrain activity from baseline to follow-up correlated with reduced simulated cocaine choice, indicating that heightened midbrain activations in this context may be marking lower approach motivation for cocaine. Normalization of midbrain function at follow-up was also suggested by exploratory comparisons with active cocaine users and healthy controls (who were assessed only at baseline). Enhanced self-control at follow-up was suggested by a trend for the commonly hypoactive dorsal anterior cingulate cortex to increase response during a drug-related context. Together, these results suggest that fMRI could be useful in sensitively tracking follow-up outcomes in drug addiction. C1 [Moeller, Scott J.; Woicik, Patricia A.; Maloney, Thomas; Alia-Klein, Nelly; Wang, Gene-Jack; Wang, Ruiliang; Bolger, Joy; Goldstein, Rita Z.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Tomasi, Dardo; Telang, Frank; Volkow, Nora D.] NIAAA, Bethesda, MD USA. [Honorio, Jean] SUNY Stony Brook, Stony Brook, NY 11794 USA. [Sinha, Rajita] Yale Univ, Sch Med, New Haven, CT USA. [Carise, Deni] Phoenix House Fdn Inc, New York, NY USA. [Carise, Deni] Univ Penn, Philadelphia, PA 19104 USA. [Astone-Twerell, Janetta] Samaritan Village Inc, Briarwood, NY USA. [Volkow, Nora D.] NIDA, Bethesda, MD 20892 USA. RP Goldstein, RZ (reprint author), Brookhaven Natl Lab, 30 Bell Ave,Bldg 490, Upton, NY 11973 USA. EM rgoldstein@bnl.gov RI Tomasi, Dardo/J-2127-2015; Moeller, Scott/L-5549-2016 OI Moeller, Scott/0000-0002-4449-0844 FU National Institute on Drug Abuse [1R01DA023579, 1F32DA030017-01]; U.S. Department of Energy [DE-AC02-98CHI-886] FX This study was supported by grants from the National Institute on Drug Abuse (to R.Z.G.: 1R01DA023579; to S.J.M.: 1F32DA030017-01).; Notice: This manuscript has been authored by Brookhaven Science Associates, LLC, under Contract No. DE-AC02-98CHI-886 with the U.S. Department of Energy. The United States Government retains, and the publisher, by accepting the article for publication, acknowledges, a world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for the United States Government purposes. NR 65 TC 18 Z9 18 U1 2 U2 6 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1355-6215 J9 ADDICT BIOL JI Addict. Biol. PD NOV PY 2012 VL 17 IS 6 BP 1013 EP 1025 DI 10.1111/j.1369-1600.2012.00440.x PG 13 WC Biochemistry & Molecular Biology; Substance Abuse SC Biochemistry & Molecular Biology; Substance Abuse GA 023UY UT WOS:000310063100008 PM 22458423 ER PT J AU Benyahia, S AF Benyahia, Sofiane TI Fine-grid simulations of gas-solids flow in a circulating fluidized bed SO AICHE JOURNAL LA English DT Article DE circulating fluidized beds; computational fluid dynamics (CFD); fluidization; multiphase flow; particle technology ID MODEL C1 Natl Energy Technol Lab, Morgantown, WV 26507 USA. RP Benyahia, S (reprint author), Natl Energy Technol Lab, Morgantown, WV 26507 USA. EM sofiane.benyahia@netl.doe.gov NR 8 TC 15 Z9 17 U1 0 U2 32 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0001-1541 J9 AICHE J JI AICHE J. PD NOV PY 2012 VL 58 IS 11 BP 3589 EP 3592 DI 10.1002/aic.13826 PG 4 WC Engineering, Chemical SC Engineering GA 017NB UT WOS:000309595600028 ER PT J AU Carter, MW Bergdall, AR Henry-Moss, D Hatfield-Timajchy, K Hock-Long, L AF Carter, Marion W. Bergdall, Anna R. Henry-Moss, Dare Hatfield-Timajchy, Kendra Hock-Long, Linda TI A qualitative study of contraceptive understanding among young adults SO CONTRACEPTION LA English DT Article DE Contraception; Young adults; Knowledge; Attitudes; Qualitative ID REPRODUCTIVE HEALTH; DECISION-MAKING; HORMONAL CONTRACEPTIVES; CONSPIRACY BELIEFS; AFRICAN-AMERICANS; UNITED-STATES; BIRTH-CONTROL; WOMEN; BARRIERS; DISPARITIES AB Background: This study describes contraceptive understanding, sources of information and consequences of contraceptive misunderstandings among urban, young adults. Study Design: We used qualitative data from 16 focus groups and 53 interviews with Puerto Rican and African American men and women aged 18-25 years from Philadelphia and Hartford. We categorized and compared assertions made about all contraceptive methods' side effects, effectiveness and use using an iterative process. Results: Participants considered contraceptive use worthwhile but felt that it carried risks of problematic side effects and contraceptive failure, with variation among methods. Men knew most about condoms and withdrawal and trusted both more than women. Personal or second-hand experience was the dominant source of information on contraceptive understanding. Misunderstandings about contraception affected their relationships and risk of unintended pregnancy. Conclusion: Contraceptive understanding is a powerful determinant of contraceptive use and limits the options perceived by young adults to prevent pregnancy. Research is needed to strengthen contraceptive counseling and outreach in ways that better leverage peer influence. Published by Elsevier Inc. C1 [Carter, Marion W.; Hatfield-Timajchy, Kendra] Ctr Dis Control & Prevent, Atlanta, GA USA. [Bergdall, Anna R.] Oak Ridge Inst Sci Educ, Oak Ridge, TN USA. [Henry-Moss, Dare; Hock-Long, Linda] Family Planning Council, Philadelphia, PA USA. RP Carter, MW (reprint author), Ctr Dis Control, 4770 Buford Highway,MS K-34, Atlanta, GA 30341 USA. EM Acq0@cdc.gov OI HENRY-MOSS, DARE/0000-0002-4088-0028 FU CDC FX There was no funding for this study. There was funding from CDC for the original data collection. NR 30 TC 9 Z9 9 U1 1 U2 26 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 0010-7824 J9 CONTRACEPTION JI Contraception PD NOV PY 2012 VL 86 IS 5 BP 543 EP 550 DI 10.1016/j.contraception.2012.02.017 PG 8 WC Obstetrics & Gynecology SC Obstetrics & Gynecology GA 022HL UT WOS:000309948500019 PM 22464411 ER PT J AU Montagner, JP Larmat, C Capdeville, Y Fink, M Phung, H Romanowicz, B Clevede, E Kawakatsu, H AF Montagner, J. -P. Larmat, C. Capdeville, Y. Fink, M. Phung, H. Romanowicz, B. Clevede, E. Kawakatsu, H. TI Time-reversal method and cross-correlation techniques by normal mode theory: a three-point problem SO GEOPHYSICAL JOURNAL INTERNATIONAL LA English DT Article DE Time series analysis; Numerical solutions; Interferometry; Earthquake source observations; Surface wave and free oscillations; Theoretical seismology ID BACKGROUND FREE OSCILLATIONS; SURFACE-WAVE TOMOGRAPHY; GREENS-FUNCTION; EARTH MODEL; SEISMIC INTERFEROMETRY; CHAOTIC CAVITIES; DIFFUSE FIELD; EXCITATION; ACOUSTICS; NOISE AB Since its beginning in acoustics, the Time-Reversal method (hereafter referred as TR) has been explored by different studies to locate and characterize seismic sources in elastic media. But few authors have proposed an analytical analysis of the method, especially in the case of an elastic medium and for a finite body such as the Earth. In this paper, we use a normal mode approach (for general 3-D case and degenerate modes in 1-D reference model) to investigate the convergence properties of the TR method. We first investigate a three-point problem, with two fixed points which are the source and the receiver and a third one corresponding to a changing observation point. We extend the problem of a single channel TR experiment to a multiple channel and multiple station TR experiment. We show as well how this problem relates to the retrieval of Greens function with a multiple source cross-correlation and also the differences between TR method and cross-correlation techniques. Since most of the noise sources are located close to the surface of the Earth, we show that the time derivative of the cross-correlation of long-period seismograms with multiple sources at the surface is different from the Greens function. Next, we show the importance of a correct surface-area weighting of the signal resent by the stations according to a Voronoi tessellation of the Earth surface. We use arguments based on the stationary phase approximation to argue that phase-information is more important than amplitude information for getting a good focusing in TR experiment. Finally, by using linear relationships between the time-reversed displacement (resp. strain wavefields) and the components of a vector force source (resp. a moment tensor source), we show how to retrieve force (or moment tensor components) of any long period tectonic or environmental sources by time reversal. C1 [Montagner, J. -P.; Capdeville, Y.; Phung, H.; Clevede, E.] CNRS, Seismol Lab, Inst Phys Globe, UMR 7154, F-75238 Paris 05, France. [Larmat, C.] LANL, Los Alamos, NM USA. [Fink, M.] CNRS, ESPCI ParisTech, Inst Langevin, F-75005 Paris, France. [Romanowicz, B.] Univ Calif Berkeley, Seismol Lab, Berkeley, CA USA. [Kawakatsu, H.] Univ Tokyo, Earthquake Res Inst, Tokyo 113, Japan. RP Montagner, JP (reprint author), CNRS, Seismol Lab, Inst Phys Globe, UMR 7154, 1 Rue Jussieu, F-75238 Paris 05, France. EM jpm@ipgp.fr RI fink, mathias/M-9437-2016; Montagner, Jean-Paul/A-8733-2011; OI Montagner, Jean-Paul/0000-0001-9958-3012; Larmat, Carene S/0000-0002-3607-7558; romanowicz, Barbara/0000-0002-6208-6044; Fink, Mathias/0000-0002-8494-7562 FU Los Alamos National Laboratory FX A number of colleagues and students have helped with suggestions for the improvement of this material. The work of Carene Larmat was partially funded by Institutional Support at Los Alamos National Laboratory, and Jean-Paul Montagner benefitted from an invitation from the Earthquake Research Institute of Tokyo and of the European ITN QUEST. NR 57 TC 2 Z9 2 U1 1 U2 25 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0956-540X EI 1365-246X J9 GEOPHYS J INT JI Geophys. J. Int. PD NOV PY 2012 VL 191 IS 2 BP 637 EP 652 DI 10.1111/j.1365-246X.2012.05619.x PG 16 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA 019QG UT WOS:000309753800020 ER PT J AU Campbell, JH Foster, CM Vishnivetskaya, T Campbell, AG Yang, ZMK Wymore, A Palumbo, AV Chesler, EJ Podar, M AF Campbell, James H. Foster, Carmen M. Vishnivetskaya, Tatiana Campbell, Alisha G. Yang, Zamin K. Wymore, Ann Palumbo, Anthony V. Chesler, Elissa J. Podar, Mircea TI Host genetic and environmental effects on mouse intestinal microbiota SO ISME JOURNAL LA English DT Article DE Collaborative Cross; intestinal microbial diversity; microbiome; microbiota; pyrosequencing; SSU rRNA gene ID GUT MICROBIOTA; COLLABORATIVE CROSS; SYSTEMS GENETICS; MICE; RESOURCE; ZEBRAFISH; DIVERSITY; PROFILES; BACTERIA; INFANT AB The mammalian gut harbors complex and variable microbial communities, across both host phylogenetic space and conspecific individuals. A synergy of host genetic and environmental factors shape these communities and account for their variability, but their individual contributions and the selective pressures involved are still not well understood. We employed barcoded pyrosequencing of V1-2 and V4 regions of bacterial small subunit ribosomal RNA genes to characterize the effects of host genetics and environment on cecum assemblages in 10 genetically distinct, inbred mouse strains. Eight of these strains are the foundation of the Collaborative Cross (CC), a panel of mice derived from a genetically diverse set of inbred founder strains, designed specifically for complex trait analysis. Diversity of gut microbiota was characterized by complementing phylogenetic and distance-based, sequence-clustering approaches. Significant correlations were found between the mouse strains and their gut microbiota, reflected by distinct bacterial communities. Cohabitation and litter had a reduced, although detectable effect, and the microbiota response to these factors varied by strain. We identified bacterial phylotypes that appear to be discriminative and strain-specific to each mouse line used. Cohabitation of different strains of mice revealed an interaction of host genetic and environmental factors in shaping gut bacterial consortia, in which bacterial communities became more similar but retained strain specificity. This study provides a baseline analysis of intestinal bacterial communities in the eight CC progenitor strains and will be linked to integrated host genotype, phenotype and microbiota research on the resulting CC panel. The ISME Journal (2012) 6, 2033-2044; doi: 10.1038/ismej.2012.54; published online 14 June 2012 C1 [Campbell, James H.; Foster, Carmen M.; Vishnivetskaya, Tatiana; Campbell, Alisha G.; Yang, Zamin K.; Wymore, Ann; Palumbo, Anthony V.; Podar, Mircea] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. [Vishnivetskaya, Tatiana] Univ Tennessee, Ctr Environm Biotechnol, Knoxville, TN 37932 USA. [Campbell, Alisha G.; Chesler, Elissa J.; Podar, Mircea] Univ Tennessee, Grad Sch Genome Sci & Technol, Knoxville, TN USA. [Chesler, Elissa J.] Jackson Lab, Bar Harbor, ME 04609 USA. RP Podar, M (reprint author), Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN 37831 USA. EM podarm@ornl.gov RI Palumbo, Anthony/A-4764-2011; Vishnivetskaya, Tatiana/A-4488-2008; OI Palumbo, Anthony/0000-0002-1102-3975; Vishnivetskaya, Tatiana/0000-0002-0660-023X; Podar, Mircea/0000-0003-2776-0205 FU US Department of Energy Office of Science, Biological and Environmental Research programs at Oak Ridge National Laboratory (ORNL); Laboratory Directed Research and Development Program of ORNL; National Human Genome Research Institute [NIH R01-HG004857]; UT-Battelle, LLC [DE-AC05-00OR22725] FX We thank J Mosher, MShakya, C Brandt, C Schadt (ORNL), M Hauser and J Becker (UTK) for many helpful discussions during data collection and analysis. We also thank L Miller (ORNL) for molecular biology assistance. We are also grateful to P Schloss (mothur; University of Michigan) and R Knight (UniFrac; University of Colorado) for guidance with their respective analytical tools. We also thank F Bushman (University of Pennsylvania) for critical evaluation of the manuscript and anonymous reviewers for helpful suggestions. This research was funded by the US Department of Energy Office of Science, Biological and Environmental Research programs at Oak Ridge National Laboratory (ORNL), by the Laboratory Directed Research and Development Program of ORNL and in part by a grant to MP from the National Human Genome Research Institute (NIH R01-HG004857). ORNL is managed by UT-Battelle, LLC, for the US Department of Energy under contract DE-AC05-00OR22725. NR 46 TC 55 Z9 56 U1 4 U2 45 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1751-7362 J9 ISME J JI ISME J. PD NOV PY 2012 VL 6 IS 11 BP 2033 EP 2044 DI 10.1038/ismej.2012.54 PG 12 WC Ecology; Microbiology SC Environmental Sciences & Ecology; Microbiology GA 023ST UT WOS:000310056400006 PM 22695862 ER PT J AU Walker, CB Redding-Johanson, AM Baidoo, EE Rajeev, L He, ZL Hendrickson, EL Joachimiak, MP Stolyar, S Arkin, AP Leigh, JA Zhou, JZ Keasling, JD Mukhopadhyay, A Stahl, DA AF Walker, Christopher B. Redding-Johanson, Alyssa M. Baidoo, Edward E. Rajeev, Lara He, Zhili Hendrickson, Erik L. Joachimiak, Marcin P. Stolyar, Sergey Arkin, Adam P. Leigh, John A. Zhou, Jizhong Keasling, Jay D. Mukhopadhyay, Aindrila Stahl, David A. TI Functional responses of methanogenic archaea to syntrophic growth SO ISME JOURNAL LA English DT Article DE methanogen; syntrophy; coculture; alanine utilization; sulfate-reducing bacteria ID DESULFOVIBRIO-VULGARIS HILDENBOROUGH; THERMOAUTOTROPHICUM DELTA-H; METHANOCOCCUS-MARIPALUDIS; METHANOBACTERIUM-THERMOAUTOTROPHICUM; DEPENDENT TRANSCRIPTION; FORMATE DEHYDROGENASE; ELECTRON-TRANSFER; GENOME SEQUENCE; SELENIUM-FREE; GENES AB Methanococcus maripaludis grown syntrophically with Desulfovibrio vulgaris was compared with M. maripaludis monocultures grown under hydrogen limitation using transcriptional, proteomic and metabolite analyses. These measurements indicate a decrease in transcript abundance for energy-consuming biosynthetic functions in syntrophically grown M. maripaludis, with an increase in transcript abundance for genes involved in the energy-generating central pathway for methanogenesis. Compared with growth in monoculture under hydrogen limitation, the response of paralogous genes, such as those coding for hydrogenases, often diverged, with transcripts of one variant increasing in relative abundance, whereas the other was little changed or significantly decreased in abundance. A common theme was an apparent increase in transcripts for functions using H-2 directly as reductant, versus those using the reduced deazaflavin (coenzyme F-420). The greater importance of direct reduction by H-2 was supported by improved syntrophic growth of a deletion mutant in an F-420-dependent dehydrogenase of M. maripaludis. These data suggest that paralogous genes enable the methanogen to adapt to changing substrate availability, sustaining it under environmental conditions that are often near the thermodynamic threshold for growth. Additionally, the discovery of interspecies alanine transfer adds another metabolic dimension to this environmentally relevant mutualism. The ISME Journal (2012) 6, 2045-2055; doi:10.1038/ismej.2012.60; published online 28 June 2012 C1 [Redding-Johanson, Alyssa M.; Baidoo, Edward E.; Rajeev, Lara; Joachimiak, Marcin P.; Arkin, Adam P.; Keasling, Jay D.; Mukhopadhyay, Aindrila] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Walker, Christopher B.; Stolyar, Sergey; Stahl, David A.] Univ Washington, Dept Civil & Environm Engn, Seattle, WA 98195 USA. [Walker, Christopher B.] Geosyntec Consultants, Seattle, WA USA. [He, Zhili; Zhou, Jizhong] Univ Oklahoma, Dept Bot & Microbiol, Norman, OK 73019 USA. [Hendrickson, Erik L.; Leigh, John A.] Univ Washington, Dept Microbiol, Seattle, WA 98195 USA. RP Mukhopadhyay, A (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, 1 Cyclotron Rd,MS 978, Berkeley, CA 94720 USA. EM amukhopadhyay@lbl.gov RI Keasling, Jay/J-9162-2012; Arkin, Adam/A-6751-2008; OI Keasling, Jay/0000-0003-4170-6088; Arkin, Adam/0000-0002-4999-2931; Rajeev, Lara/0000-0002-0106-9195 FU US Department of Energy, Office of Science, Office of Biological and Environmental Research, Genomics: GTL Foundational Science [DE-AC0205CH11231]; Lawrence Berkeley National Laboratory; US Department of Energy FX We thank Professor Michael J McInerney (University of Okhlahoma) for valuable discussion and review of an earlier draft of this paper, Dr Christopher Petzold (LBNL) for help with iTRAQ data analysis on Protein Pilot and Jason Baumohl (LBNL) for help with submitting data to the GEO database. This work is part of ENIGMA, a Scientific Focus Area Program supported by the US Department of Energy, Office of Science, Office of Biological and Environmental Research, Genomics: GTL Foundational Science through contract DE-AC0205CH11231 between Lawrence Berkeley National Laboratory and the US Department of Energy. NR 37 TC 21 Z9 22 U1 4 U2 75 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1751-7362 J9 ISME J JI ISME J. PD NOV PY 2012 VL 6 IS 11 BP 2045 EP 2055 DI 10.1038/ismej.2012.60 PG 11 WC Ecology; Microbiology SC Environmental Sciences & Ecology; Microbiology GA 023ST UT WOS:000310056400007 PM 22739494 ER PT J AU Reith, F Brugger, J Zammit, CM Gregg, AL Goldfarb, KC Andersen, GL DeSantis, TZ Piceno, YM Brodie, EL Lu, ZM He, ZL Zhou, JZ Wakelin, SA AF Reith, Frank Brugger, Joel Zammit, Carla M. Gregg, Adrienne L. Goldfarb, Katherine C. Andersen, Gary L. DeSantis, Todd Z. Piceno, Yvette M. Brodie, Eoin L. Lu, Zhenmei He, Zhili Zhou, Jizhong Wakelin, Steven A. TI Influence of geogenic factors on microbial communities in metallogenic Australian soils SO ISME JOURNAL LA English DT Article DE soil; landform; bacteria; gold; microarray; Australia ID ACID-MINE DRAINAGE; NEW-SOUTH-WALES; PARK GOLD MINE; BACTERIAL COMMUNITIES; LAND-USE; DIVERSITY; MICROARRAY; BIOMINERALIZATION; POPULATIONS; PATTERNS AB Links between microbial community assemblages and geogenic factors were assessed in 187 soil samples collected from four metal-rich provinces across Australia. Field-fresh soils and soils incubated with soluble Au(III) complexes were analysed using three-domain multiplex-terminal restriction fragment length polymorphism, and phylogenetic (PhyloChip) and functional (GeoChip) microarrays. Geogenic factors of soils were determined using lithological-, geomorphological- and soil-mapping combined with analyses of 51 geochemical parameters. Microbial communities differed significantly between landforms, soil horizons, lithologies and also with the occurrence of underlying Au deposits. The strongest responses to these factors, and to amendment with soluble Au(III) complexes, was observed in bacterial communities. PhyloChip analyses revealed a greater abundance and diversity of Alphaproteobacteria (especially Sphingomonas spp.), and Firmicutes (Bacillus spp.) in Au-containing and Au(III)-amended soils. Analyses of potential function (GeoChip) revealed higher abundances of metal-resistance genes in metal-rich soils. For example, genes that hybridised with metal-resistance genes copA, chrA and czcA of a prevalent aurophillic bacterium, Cupriavidus metallidurans CH34, occurred only in auriferous soils. These data help establish key links between geogenic factors and the phylogeny and function within soil microbial communities. In particular, the landform, which is a crucial factor in determining soil geochemistry, strongly affected microbial community structures. The ISME Journal (2012) 6, 2107-2118; doi:10.1038/ismej.2012.48; published online 7 June 2012 C1 [Reith, Frank; Brugger, Joel; Zammit, Carla M.] Univ Adelaide, Ctr Tecton Resources & Mineral Explorat TRaX, Sch Earth & Environm Sci, Adelaide, SA, Australia. [Reith, Frank; Zammit, Carla M.; Gregg, Adrienne L.] CSIRO Land & Water, Environm Biogeochem, PMB2, Glen Osmond, SA 5064, Australia. [Brugger, Joel] S Australian Museum, Dept Mineral, Adelaide, SA 5000, Australia. [Goldfarb, Katherine C.; Andersen, Gary L.; DeSantis, Todd Z.; Piceno, Yvette M.; Brodie, Eoin L.] Lawrence Berkeley Natl Lab, Dept Ecol, Div Earth Sci, Berkeley, CA USA. [Lu, Zhenmei] Zhejang Univ, Coll Life Sci, Hangzhou, Zhejiang, Peoples R China. [Lu, Zhenmei; He, Zhili; Zhou, Jizhong] Univ Oklahoma, Inst Environm Genom, Norma, OK USA. [Lu, Zhenmei; He, Zhili; Zhou, Jizhong] Univ Oklahoma, Dept Bot & Microbiol, Norma, OK USA. [Wakelin, Steven A.] AgResearch Ltd, Lincoln Sci Ctr, Christchurch, New Zealand. RP Reith, F (reprint author), Univ Adelaide, Ctr Tecton Resources & Mineral Explorat TRaX, Sch Earth & Environm Sci, Adelaide, SA, Australia. EM Frank.Reith@csiro.au RI Wakelin, Steven/C-3170-2011; Andersen, Gary/G-2792-2015; Zammit, Carla/D-9306-2014; Brodie, Eoin/A-7853-2008; Piceno, Yvette/I-6738-2016; Brugger, Joel/C-7113-2008 OI Wakelin, Steven/0000-0002-1167-8699; Andersen, Gary/0000-0002-1618-9827; Brodie, Eoin/0000-0002-8453-8435; Piceno, Yvette/0000-0002-7915-4699; Brugger, Joel/0000-0003-1510-5764 FU Australian Research Council [LP100200212]; CSIRO Land and Water; University of Adelaide; Barrick Gold of Australia Limited; Institute for Mineral and Energy Resources; Centre for Tectonics, Resources and Exploration (TRAX) [214]; US Department Energy [DE-AC02-5CH11231, DE-SC0004601]; Newmont Exploration Pty Ltd FX We acknowledge the Australian Research Council (LP100200212 to FR), CSIRO Land and Water, The University of Adelaide, Newmont Exploration Pty Ltd, Barrick Gold of Australia Limited, Institute for Mineral and Energy Resources and the Centre for Tectonics, Resources and Exploration (TRAX no. 214), US Department Energy (DE-AC02-5CH11231 and DE-SC0004601). We thank L Fairbrother, C Wright for assistance with analyses, the editor IM Head and the anonymous reviewers for their suggestions. NR 45 TC 17 Z9 17 U1 5 U2 56 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1751-7362 J9 ISME J JI ISME J. PD NOV PY 2012 VL 6 IS 11 BP 2107 EP 2118 DI 10.1038/ismej.2012.48 PG 12 WC Ecology; Microbiology SC Environmental Sciences & Ecology; Microbiology GA 023ST UT WOS:000310056400012 PM 22673626 ER PT J AU Rajeev, L Hillesland, KL Zane, GM Zhou, AF Joachimiak, MP He, ZL Zhou, JZ Arkin, AP Wall, JD Stahl, DA AF Rajeev, Lara Hillesland, Kristina L. Zane, Grant M. Zhou, Aifen Joachimiak, Marcin P. He, Zhili Zhou, Jizhong Arkin, Adam P. Wall, Judy D. Stahl, David A. TI Deletion of the Desulfovibrio vulgaris Carbon Monoxide Sensor Invokes Global Changes in Transcription SO JOURNAL OF BACTERIOLOGY LA English DT Article ID SULFATE-REDUCING BACTERIA; REGULATOR FUR MUTANT; RHODOSPIRILLUM-RUBRUM; OXIDATIVE STRESS; PHYSIOLOGICAL-FUNCTION; HILDENBOROUGH; HYDROGEN; METABOLISM; SYSTEM; DEHYDROGENASE AB The carbon monoxide-sensing transcriptional factor CooA has been studied only in hydrogenogenic organisms that can grow using CO as the sole source of energy. Homologs for the canonical CO oxidation system, including CooA, CO dehydrogenase (CODH), and a CO-dependent Coo hydrogenase, are present in the sulfate-reducing bacterium Desulfovibrio vulgaris, although it grows only poorly on CO. We show that D. vulgaris Hildenborough has an active CO dehydrogenase capable of consuming exogenous CO and that the expression of the CO dehydrogenase, but not that of a gene annotated as encoding a Coo hydrogenase, is dependent on both CO and CooA. Carbon monoxide did not act as a general metabolic inhibitor, since growth of a strain deleted for cooA was inhibited by CO on lactate-sulfate but not pyruvate-sulfate. While the deletion strain did not accumulate CO in excess, as would have been expected if CooA were important in the cycling of CO as a metabolic intermediate, global transcriptional analyses suggested that CooA and CODH are used during normal metabolism. C1 [Rajeev, Lara; Joachimiak, Marcin P.; Arkin, Adam P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Rajeev, Lara; Hillesland, Kristina L.; Stahl, David A.] Univ Washington, Dept Civil & Environm Engn, Seattle, WA 98195 USA. [Hillesland, Kristina L.] Univ Washington, Sci & Technol Program, Bothell, WA USA. [Zane, Grant M.; Wall, Judy D.] Univ Missouri, Dept Biochem, Columbia, MO USA. [Zhou, Aifen; He, Zhili; Zhou, Jizhong] Univ Oklahoma, Dept Microbiol & Plant Biol, Inst Environm Genom, Norman, OK 73019 USA. RP Rajeev, L (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. EM lrajeev@lbl.gov RI He, Zhili/C-2879-2012; Arkin, Adam/A-6751-2008; OI Arkin, Adam/0000-0002-4999-2931; Rajeev, Lara/0000-0002-0106-9195 FU Office of Science, Office of Biological and Environmental Research, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work, conducted by ENIGMA (Ecosystems and Networks Integrated with Genes and Molecular Assemblies [http://enigma.lbl.gov]), a Scientific Focus Area Program at Lawrence Berkeley National Laboratory, was supported by the Office of Science, Office of Biological and Environmental Research, of the U.S. Department of Energy, under contract no. DE-AC02-05CH11231. NR 34 TC 7 Z9 7 U1 2 U2 14 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 0021-9193 J9 J BACTERIOL JI J. Bacteriol. PD NOV PY 2012 VL 194 IS 21 BP 5783 EP 5793 DI 10.1128/JB.00749-12 PG 11 WC Microbiology SC Microbiology GA 022VB UT WOS:000309990800007 PM 22904289 ER PT J AU Reyes, C Qian, F Zhang, A Bondarev, S Welch, A Thelen, MP Saltikov, CW AF Reyes, Carolina Qian, Fang Zhang, Alissa Bondarev, Sergey Welch, Angel Thelen, Michael P. Saltikov, Chad W. TI Characterization of Axial and Proximal Histidine Mutations of the Decaheme Cytochrome MtrA from Shewanella sp Strain ANA-3 and Implications for the Electron Transport System SO JOURNAL OF BACTERIOLOGY LA English DT Article ID C-TYPE CYTOCHROMES; ONEIDENSIS MR-1; IRON REDUCTION; HEME; IDENTIFICATION; ARSENATE; LIGANDS; OMCA AB Extracellular respiration of solid-phase electron acceptors in some microorganisms requires a complex chain of multiheme c-type cytochromes that span the inner and outer membranes. In Shewanella species, MtrA, an similar to 35-kDa periplasmic decaheme c-type cytochrome, is an essential component for extracellular respiration of iron(III). The exact mechanism of electron transport has not yet been resolved, but the arrangement of the polypeptide chain may have a strong influence on the capability of the MtrA cytochrome to transport electrons. The iron hemes of MtrA are bound to its polypeptide chain via proximal (CXXCH) and distal histidine residues. In this study, we show the effects of mutating histidine residues of MtrA to arginine on protein expression and extracellular respiration using Shewanella sp. strain ANA-3 as a model organism. Individual mutations to six out of nine proximal histidines in CXXCH of MtrA led to decreased protein expression. However, distal histidine mutations resulted in various degrees of protein expression. In addition, the effects of histidine mutations on extracellular respiration were tested using ferrihydrite and current production in microbial fuel cells. These results show that proximal histidine mutants were unable to reduce ferrihydrite. Mutations to the distal histidine residues resulted in various degrees of ferrihydrite reduction. These findings indicate that mutations to the proximal histidine residues affect MtrA expression, leading to loss of extracellular respiration ability. In contrast, mutations to the distal histidine residues are less detrimental to protein expression, and extracellular respiration can proceed. C1 [Reyes, Carolina; Bondarev, Sergey; Welch, Angel; Saltikov, Chad W.] Univ Calif Santa Cruz, Dept Microbiol & Environm Toxicol, Santa Cruz, CA 95064 USA. [Qian, Fang; Zhang, Alissa] Univ Calif Santa Cruz, Dept Chem & Biochem, Santa Cruz, CA 95064 USA. [Qian, Fang; Thelen, Michael P.] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA USA. RP Saltikov, CW (reprint author), Univ Calif Santa Cruz, Dept Microbiol & Environm Toxicol, Santa Cruz, CA 95064 USA. EM creyes6@gmail.com; salitkov@ucsc.edu RI Thelen, Michael/C-6834-2008; Thelen, Michael/G-2032-2014; OI Thelen, Michael/0000-0002-2479-5480; Thelen, Michael/0000-0002-2479-5480; Reyes, Carolina/0000-0002-7413-607X FU National Science Foundation [EAR 21472-443143]; University of California, Santa Cruz, Minority Biomedical Research Support Fellowship (MBRS); Research Mentoring Institute (RMI) Graduate Diversity Fellowship; Alliance for Graduate Education and the Professoriate Program (AGEP); LDRD project [11-LW-054]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DEAC52-07NA27344] FX C.W.S. acknowledges support from National Science Foundation research grant EAR 21472-443143. C.R. was supported by a University of California, Santa Cruz, Minority Biomedical Research Support Fellowship (MBRS); a Research Mentoring Institute (RMI) Graduate Diversity Fellowship; and the Alliance for Graduate Education and the Professoriate Program (AGEP). C.R. also acknowledges Hanse Wissenschaftskolleg (HWK), Delmenhorst, Germany, for support during the preparation of the manuscript. F.Q. and M.P.T. acknowledge support from LDRD project 11-LW-054, performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under contract DEAC52-07NA27344. NR 28 TC 1 Z9 1 U1 1 U2 17 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 0021-9193 J9 J BACTERIOL JI J. Bacteriol. PD NOV PY 2012 VL 194 IS 21 BP 5840 EP 5847 DI 10.1128/JB.00890-12 PG 8 WC Microbiology SC Microbiology GA 022VB UT WOS:000309990800012 PM 22923588 ER PT J AU Desiniotis, A Kouvelis, VN Davenport, K Bruce, D Detter, C Tapia, R Han, C Goodwin, LA Woyke, T Kyrpides, NC Typas, MA Pappas, KM AF Desiniotis, Andreas Kouvelis, Vassili N. Davenport, Karen Bruce, David Detter, Chris Tapia, Roxanne Han, Cliff Goodwin, Lynne A. Woyke, Tanja Kyrpides, Nikos C. Typas, Milton A. Pappas, Katherine M. TI Complete Genome Sequence of the Ethanol-Producing Zymomonas mobilis subsp mobilis Centrotype ATCC 29191 SO JOURNAL OF BACTERIOLOGY LA English DT Article ID TOOL AB Zymomonas mobilis is an ethanologenic bacterium that has been studied for use in biofuel production. Of the sequenced Zymomonas strains, ATCC 29191 has been described as the phenotypic centrotype of Zymomonas mobilis subsp. mobilis, the taxon that harbors the highest ethanol-producing Z. mobilis strains. ATCC 29191 was isolated in Kinshasa, Congo, from palm wine fermentations. This strain is reported to be a robust levan producer, while in recent years it has been employed in studies addressing Z. mobilis respiration. Here we announce the finishing and annotation of the ATCC 29191 genome, which comprises one chromosome and three plasmids. C1 [Desiniotis, Andreas; Kouvelis, Vassili N.; Typas, Milton A.; Pappas, Katherine M.] Univ Athens, Fac Biol, Dept Genet & Biotechnol, Athens, Greece. [Davenport, Karen; Detter, Chris; Tapia, Roxanne; Han, Cliff; Goodwin, Lynne A.; Woyke, Tanja] Los Alamos Natl Lab, Biosci Div, DOE Joint Genome Inst, Los Alamos, NM USA. [Bruce, David; Kyrpides, Nikos C.] DOE Joint Genome Inst, Walnut Creek, CA USA. RP Pappas, KM (reprint author), Univ Athens, Fac Biol, Dept Genet & Biotechnol, Athens, Greece. EM kmpappas@biol.uoa.gr RI Kyrpides, Nikos/A-6305-2014 OI Kyrpides, Nikos/0000-0002-6131-0462 FU U.S. DOE Office of Science [DE-AC02-05CH11231]; NKUA Research Committee [70/4/7809]; Vienna Medical Society/Sanofi FX Work at the DOE JGI is financed by the U.S. DOE Office of Science, contract number DE-AC02-05CH11231. K.M.P. thanks the NKUA Research Committee for award 70/4/7809. A.D. thanks the Vienna Medical Society/Sanofi for the Wilhelm-Auerswald-Preis 2012 award. NR 21 TC 10 Z9 10 U1 2 U2 6 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 0021-9193 J9 J BACTERIOL JI J. Bacteriol. PD NOV PY 2012 VL 194 IS 21 BP 5966 EP 5967 DI 10.1128/JB.01398-12 PG 2 WC Microbiology SC Microbiology GA 022VB UT WOS:000309990800028 PM 23045486 ER PT J AU Lucas, S Han, J Lapidus, A Cheng, JF Goodwin, LA Pitluck, S Peters, L Mikhailova, N Teshima, H Detter, JC Han, C Tapia, R Land, M Hauser, L Kyrpides, NC Ivanova, N Pagani, I Vannier, P Oger, P Bartlett, DH Noll, KM Woyke, T Jebbar, M AF Lucas, Susan Han, James Lapidus, Alla Cheng, Jan-Fang Goodwin, Lynne A. Pitluck, Sam Peters, Lin Mikhailova, Natalia Teshima, Hazuki Detter, John C. Han, Cliff Tapia, Roxanne Land, Miriam Hauser, Loren Kyrpides, Nikos C. Ivanova, Natalia Pagani, Ioanna Vannier, Pauline Oger, Phil Bartlett, Douglas H. Noll, Kenneth M. Woyke, Tanja Jebbar, Mohamed TI Complete Genome Sequence of the Thermophilic, Piezophilic, Heterotrophic Bacterium Marinitoga piezophila KA3 SO JOURNAL OF BACTERIOLOGY LA English DT Article ID SEA HYDROTHERMAL VENT; SP-NOV.; ORDER THERMOTOGALES AB Marinitoga piezophila KA3 is a thermophilic, anaerobic, chemoorganotrophic, sulfur-reducing bacterium isolated from the Grandbonum deep-sea hydrothermal vent site at the East Pacific Rise (13 degrees N, 2,630-m depth). The genome of M. piezophila KA3 comprises a 2,231,407-bp circular chromosome and a 13,386-bp circular plasmid. This genome was sequenced within Department of Energy Joint Genome Institute CSP 2010. C1 [Vannier, Pauline; Jebbar, Mohamed] UBO, IUEM, UMR 6197, Plouzane, France. [Lucas, Susan; Han, James; Lapidus, Alla; Cheng, Jan-Fang; Goodwin, Lynne A.; Pitluck, Sam; Peters, Lin; Mikhailova, Natalia; Detter, John C.; Han, Cliff; Tapia, Roxanne; Land, Miriam; Hauser, Loren; Kyrpides, Nikos C.; Ivanova, Natalia; Pagani, Ioanna; Woyke, Tanja] DOE Joint Genome Inst, Walnut Creek, CA USA. [Goodwin, Lynne A.; Teshima, Hazuki; Detter, John C.; Han, Cliff; Tapia, Roxanne] Los Alamos Natl Lab, Biosci Div, Los Alamos, NM USA. [Land, Miriam; Hauser, Loren] Oak Ridge Natl Lab, Oak Ridge, TN USA. [Vannier, Pauline; Jebbar, Mohamed] CNRS, IUEM, UMR 6197, Plouzane, France. [Oger, Phil] CNRS, Lab Sci Terre, UMR 5570, Lyon, France. [Oger, Phil] Univ Lyon, Lab Sci Terre, Ecole Normale Super Lyon, Lyon, France. [Bartlett, Douglas H.] Univ Calif San Diego, Scripps Inst Oceanog, Div Marine Biol Res, La Jolla, CA 92093 USA. [Noll, Kenneth M.] Univ Connecticut, Dept Mol & Cell Biol, Storrs, CT USA. RP Jebbar, M (reprint author), UBO, IUEM, UMR 6197, Technopole Brest Iroise, Plouzane, France. EM Mohamed.Jebbar@univ-brest.fr RI Pagani, Ioanna/E-7390-2012; Lapidus, Alla/I-4348-2013; Land, Miriam/A-6200-2011; Oger, Phil/C-8138-2012; Kyrpides, Nikos/A-6305-2014; Jebbar, Mohamed/F-8597-2015 OI Lapidus, Alla/0000-0003-0427-8731; Land, Miriam/0000-0001-7102-0031; Oger, Phil/0000-0001-6298-6870; Kyrpides, Nikos/0000-0002-6131-0462; Jebbar, Mohamed/0000-0003-3879-4400 FU Agence Nationale de la Recherche [ANR-10-BLAN-Living Deep]; Ministere de l'Enseignement Superieur et de la Recherche; Office of Science of the U.S. DOE FX This work was supported in part by the Agence Nationale de la Recherche (ANR-10-BLAN-Living Deep). P.V. was supported by a Ph.D. fellowship from the Ministere de l'Enseignement Superieur et de la Recherche. The work that was conducted by the U.S. DOE JGI was supported by the Office of Science of the U.S. DOE. NR 7 TC 7 Z9 8 U1 2 U2 21 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 0021-9193 J9 J BACTERIOL JI J. Bacteriol. PD NOV PY 2012 VL 194 IS 21 BP 5974 EP 5975 DI 10.1128/JB.01430-12 PG 2 WC Microbiology SC Microbiology GA 022VB UT WOS:000309990800033 PM 23045491 ER PT J AU Brown, SD Utturkar, SM Klingeman, DM Johnson, CM Martin, SL Land, ML Lu, TYS Schadt, CW Doktycz, MJ Pelletier, DA AF Brown, Steven D. Utturkar, Sagar M. Klingeman, Dawn M. Johnson, Courtney M. Martin, Stanton L. Land, Miriam L. Lu, Tse-Yuan S. Schadt, Christopher W. Doktycz, Mitchel J. Pelletier, Dale A. TI Twenty-One Genome Sequences from Pseudomonas Species and 19 Genome Sequences from Diverse Bacteria Isolated from the Rhizosphere and Endosphere of Populus deltoides SO JOURNAL OF BACTERIOLOGY LA English DT Article ID GROWTH-PROMOTING BACTERIUM; CONTAINS; STRAINS; PLANTS; ROOT AB To aid in the investigation of the Populus deltoides microbiome, we generated draft genome sequences for 21 Pseudomonas strains and 19 other diverse bacteria isolated from Populus deltoides roots. Genome sequences for isolates similar to Acidovorax, Bradyrhizobium, Brevi bacillus, Caulobacter, Chryseobacterium, Flavobacteriutn, Herbaspirillum, Novosphingobium, Pantoea, Phyllobacterium, Polaromonas, Rhizobium, Sphingobium, and Variovorax were generated. C1 [Brown, Steven D.; Klingeman, Dawn M.; Johnson, Courtney M.; Land, Miriam L.; Lu, Tse-Yuan S.; Schadt, Christopher W.; Doktycz, Mitchel J.; Pelletier, Dale A.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN USA. [Brown, Steven D.; Utturkar, Sagar M.; Schadt, Christopher W.; Doktycz, Mitchel J.; Pelletier, Dale A.] Univ Tennessee, Grad Sch Genome Sci & Technol, Knoxville, TN USA. [Martin, Stanton L.] N Carolina State Univ, Raleigh, NC 27695 USA. RP Brown, SD (reprint author), Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN USA. EM brownsd@ornl.gov; pelletierda@ornl.gov RI Schadt, Christopher/B-7143-2008; Doktycz, Mitchel/A-7499-2011; Land, Miriam/A-6200-2011; Klingeman, Dawn/B-9415-2012; OI Schadt, Christopher/0000-0001-8759-2448; Doktycz, Mitchel/0000-0003-4856-8343; Land, Miriam/0000-0001-7102-0031; Utturkar, Sagar/0000-0002-3453-1948; Klingeman, Dawn/0000-0002-4307-2560; Brown, Steven/0000-0002-9281-3898 FU Genomic Science Program, U.S. Department of Energy, Office of Science, Biological and Environmental Research, as part of the Plant Microbe Interfaces Scientific Focus Area; U.S. Department of Energy [DE-AC05-00OR22725] FX This research was sponsored by the Genomic Science Program, U.S. Department of Energy, Office of Science, Biological and Environmental Research, as part of the Plant Microbe Interfaces Scientific Focus Area (http://pmi.ornl.gov). Oak Ridge National Laboratory is managed by UT-Battelle LLC, for the U.S. Department of Energy under contract DE-AC05-00OR22725. NR 27 TC 58 Z9 59 U1 1 U2 58 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 0021-9193 J9 J BACTERIOL JI J. Bacteriol. PD NOV PY 2012 VL 194 IS 21 BP 5991 EP 5993 DI 10.1128/JB.01243-12 PG 3 WC Microbiology SC Microbiology GA 022VB UT WOS:000309990800043 PM 23045501 ER PT J AU Quiros-Alcala, L Bradman, A Smith, K Weerasekera, G Odetokun, M Barr, DB Nishioka, M Castorina, R Hubbard, AE Nicas, M Hammond, SK McKone, TE Eskenazi, B AF Quiros-Alcala, Lesliam Bradman, Asa Smith, Kimberly Weerasekera, Gayanga Odetokun, Martins Barr, Dana Boyd Nishioka, Marcia Castorina, Rosemary Hubbard, Alan E. Nicas, Mark Hammond, S. Katharine McKone, Thomas E. Eskenazi, Brenda TI Organophosphorous pesticide breakdown products in house dust and children's urine SO JOURNAL OF EXPOSURE SCIENCE AND ENVIRONMENTAL EPIDEMIOLOGY LA English DT Article DE biomarkers; dialkylphosphates; dust; metabolites; organophosphates; urine ID MEXICAN-AMERICAN CHILDREN; AGRICULTURAL COMMUNITY; RISK-ASSESSMENT; EXPOSURE; CHLORPYRIFOS; 3,5,6-TRICHLORO-2-PYRIDINOL; ASSESSMENTS; METABOLITES; CHAMACOS; COHORT AB Human exposure to preformed dialkylphosphates (DAPs) in food or the environment may affect the reliability of DAP urinary metabolites as biomarkers of organophosphate (OP) pesticide exposure. We conducted a study to investigate the presence of DAPs in indoor residential environments and their association with children's urinary DAP levels. We collected dust samples from homes in farmworker and urban communities (40 homes total, n = 79 samples) and up to two urine samples from resident children ages 3-6 years. We measured six DAPs in all samples and eight DAP-devolving OP pesticides in a subset of dust samples (n = 54). DAPs were detected in dust with diethylphosphate (DEP) being the most frequently detected (>= 60%); detection frequencies for other DAPs were <= 50%. DEP dust concentrations did not significantly differ between communities, nor were concentrations significantly correlated with concentrations of chlorpyrifos and diazinon, the most frequently detected diethyl-OP pesticides (Spearman rho = -0.41 to 0.38, P > 0.05). Detection of DEP, chlorpyrifos, or diazinon, was not associated with DEP and/or DEP + diethylthiophosphate detection in urine (Kappa coefficients = -0.33 to 0.16). Finally, estimated non-dietary ingestion intake from DEP in dust was found to be <= 5% of the dose calculated from DEP levels in urine, suggesting that ingestion of dust is not a significant source of DAPs in urine if they are excreted unchanged. C1 [Quiros-Alcala, Lesliam; Bradman, Asa; Castorina, Rosemary; McKone, Thomas E.; Eskenazi, Brenda] Univ Calif Berkeley, Ctr Environm Res & Childrens Hlth, Sch Publ Hlth, Berkeley, CA 94704 USA. [Quiros-Alcala, Lesliam] US EPA, EPA STAR, Washington, DC 20460 USA. [Smith, Kimberly; Weerasekera, Gayanga; Odetokun, Martins] Ctr Dis Control & Prevent, Natl Ctr Environm Hlth, Atlanta, GA USA. [Barr, Dana Boyd] Emory Univ, Rollins Sch Publ Hlth, Atlanta, GA 30322 USA. [Nishioka, Marcia] Battelle Mem Inst, Columbus, OH 43201 USA. [Hubbard, Alan E.] Univ Calif Berkeley, Sch Publ Hlth, Div Biostat, Berkeley, CA 94720 USA. [Nicas, Mark; Hammond, S. Katharine] Univ Calif Berkeley, Sch Publ Hlth, Div Environm Hlth Sci, Berkeley, CA 94720 USA. [McKone, Thomas E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. RP Bradman, A (reprint author), Univ Calif Berkeley, Ctr Environm Res & Childrens Hlth, Sch Publ Hlth, 1995 Univ Ave,Suite 265, Berkeley, CA 94704 USA. EM abradman@berkeley.edu RI Barr, Dana/E-6369-2011; Barr, Dana/E-2276-2013; Quiros-Alcala, Lesliam /Q-4928-2016 OI Quiros-Alcala, Lesliam /0000-0002-6600-7227 FU EPA [RD 83171001]; NIEHS [PO1 ES009605]; EPA STAR Doctoral Fellowship [F5D30812]; University of California Institute for Mexico; United States (UC MEXUS); Center for Latino Policy Research at the University of California at Berkeley FX This work was supported by EPA (RD 83171001) and NIEHS (PO1 ES009605). Its contents are solely the responsibility of the authors and do not necessarily represent the official views of the EPA, NIEHS, or other funders. Additional support was provided by an EPA STAR Doctoral Fellowship (F5D30812), the University of California Institute for Mexico and the United States (UC MEXUS), and the Center for Latino Policy Research at the University of California at Berkeley. We thank the CHAMACOS staff, community partners including Drs. John Pescetti and Claire Horton at Clinica de la Raze for their support in recruitment efforts, our study participants, Dr. Do-Gyun Kim and Carolina Fernandez from the Pesticide Toxicology Laboratory at the CDC for their assistance with urine sample analysis, and Dr. Rosana Weldon for editorial comments. NR 31 TC 13 Z9 13 U1 3 U2 37 PU NATURE PUBLISHING GROUP PI NEW YORK PA 75 VARICK ST, 9TH FLR, NEW YORK, NY 10013-1917 USA SN 1559-0631 J9 J EXPO SCI ENV EPID JI J. Expo. Sci. Environ. Epidemiol. PD NOV-DEC PY 2012 VL 22 IS 6 BP 559 EP 568 DI 10.1038/jes.2012.46 PG 10 WC Environmental Sciences; Public, Environmental & Occupational Health; Toxicology SC Environmental Sciences & Ecology; Public, Environmental & Occupational Health; Toxicology GA 022US UT WOS:000309989900003 PM 22781438 ER PT J AU Ravel, B Hester, JR Sole, VA Newville, M AF Ravel, B. Hester, J. R. Sole, V. A. Newville, M. TI Towards data format standardization for X-ray absorption spectroscopy SO JOURNAL OF SYNCHROTRON RADIATION LA English DT Article; Proceedings Paper CT International Workshop on Improving Data Qualityand Quantity for XAFS Experiments CY APR 12-13, 2011 CL Tsukuba, JAPAN DE XAFS; standardization; data formats ID MODEL AB A working group on data format standardization for X-ray absorption spectroscopy (XAS) has recently formed under the auspices of the International X-ray Absorption Society and the XAFS Commission of the International Union of Crystallography. This group of beamline scientists and XAS practitioners has been tasked to propose data format standards to meet the needs of the world-wide XAS community. In this report, concepts for addressing three XAS data storage needs are presented: a single spectrum interchange format, a hierarchical format for multispectral X-ray experiment, and a relational database format for XAS data libraries. C1 [Ravel, B.] NIST, Gaithersburg, MD 20899 USA. [Hester, J. R.] ANSTO, Bragg Inst, Kirrawee Dc, NSW 2232, Australia. [Sole, V. A.] European Synchrotron Radiat Facil, F-38043 Grenoble 9, France. [Newville, M.] Univ Chicago, Argonne Natl Lab, Ctr Adv Radiat Studies, Argonne, IL 60439 USA. RP Ravel, B (reprint author), NIST, Gaithersburg, MD 20899 USA. EM bravel@bnl.gov NR 11 TC 9 Z9 9 U1 1 U2 26 PU INT UNION CRYSTALLOGRAPHY PI CHESTER PA 2 ABBEY SQ, CHESTER, CH1 2HU, ENGLAND SN 1600-5775 J9 J SYNCHROTRON RADIAT JI J. Synchrot. Radiat. PD NOV PY 2012 VL 19 BP 869 EP 874 DI 10.1107/S0909049512036886 PN 6 PG 6 WC Instruments & Instrumentation; Optics; Physics, Applied SC Instruments & Instrumentation; Optics; Physics GA 024ZL UT WOS:000310151000004 PM 23093744 ER PT J AU Fulton, JL Balasubramanian, M Pham, VT Deverman, GS AF Fulton, John L. Balasubramanian, Mahalingam Van-Thai Pham Deverman, George S. TI A variable ultra-short-pathlength solution cell for XAFS transmission spectroscopy of light elements SO JOURNAL OF SYNCHROTRON RADIATION LA English DT Article; Proceedings Paper CT International Workshop on Improving Data Qualityand Quantity for XAFS Experiments CY APR 12-13, 2011 CL Tsukuba, JAPAN DE X-ray absorption fine structure; XAFS; low-Z cell; short pathlength ID ABSORPTION FINE-STRUCTURE; LIQUID WATER; ELECTROLYTES; IONS AB An X-ray absorption fine-structure spectroscopy (XAFS) cell that is suitable for solution-phase studies of the light elements in the series from Na+ and Ca2+ is described. This cell has an ultra-short pathlength that can be remotely adjusted using a miniature stepper-motor drive and thereby readily provides transmission pathlengths in the range from submicrometer to several hundred micrometers. The flexibility to vary the pathlength enables acquisition of high-quality XAFS spectra and also allows one to check for potential distortions in the spectra from thickness effects. The primary components are mostly commercially available optical parts. The performance of this device is demonstrated at the Cl K-edge (2.8 keV) for several different aqueous Cl- solutions. C1 [Fulton, John L.; Van-Thai Pham] Pacific NW Natl Lab, Div Chem & Mat Sci, Richland, WA 99354 USA. [Balasubramanian, Mahalingam] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. [Deverman, George S.] Pacific NW Natl Lab, Energy Proc & Mat Div, Richland, WA 99354 USA. RP Fulton, JL (reprint author), Pacific NW Natl Lab, Div Chem & Mat Sci, Richland, WA 99354 USA. EM john.fulton@pnnl.gov FU US Department of Energy's (DOE) Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences; US Department of Energy, Basic Energy Sciences; NSERC; University of Washington; Simon Fraser University; Pacific Northwest National Laboratory; Advanced Photon Source.; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work was supported by the US Department of Energy's (DOE) Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences. PNNL is operated for the Department of Energy by Battelle. XSD/PNC facilities at the Advanced Photon Source, and research at these facilities, are supported by the US Department of Energy, Basic Energy Sciences, a major facilities access grant from NSERC, the University of Washington, Simon Fraser University, the Pacific Northwest National Laboratory and the Advanced Photon Source. Use of the Advanced Photon Source is also supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract DE-AC02-06CH11357. NR 19 TC 7 Z9 7 U1 0 U2 26 PU INT UNION CRYSTALLOGRAPHY PI CHESTER PA 2 ABBEY SQ, CHESTER, CH1 2HU, ENGLAND SN 1600-5775 J9 J SYNCHROTRON RADIAT JI J. Synchrot. Radiat. PD NOV PY 2012 VL 19 BP 949 EP 953 DI 10.1107/S090904951203806X PN 6 PG 5 WC Instruments & Instrumentation; Optics; Physics, Applied SC Instruments & Instrumentation; Optics; Physics GA 024ZL UT WOS:000310151000014 PM 23093754 ER PT J AU Leontowich, AFG Hitchcock, AP Tyliszczak, T Weigand, M Wang, J Karunakaran, C AF Leontowich, Adam F. G. Hitchcock, Adam P. Tyliszczak, Tolek Weigand, Markus Wang, Jian Karunakaran, Chithra TI Accurate dosimetry in scanning transmission X-ray microscopes via the cross-linking threshold dose of poly(methyl methacrylate) SO JOURNAL OF SYNCHROTRON RADIATION LA English DT Article; Proceedings Paper CT International Workshop on Improving Data Qualityand Quantity for XAFS Experiments CY APR 12-13, 2011 CL Tsukuba, JAPAN DE poly(methyl methacrylate); STXM; radiation damage; dosimetry; detector efficiency ID ADVANCED LIGHT-SOURCE; RADIATION-DAMAGE; POLYMETHYL METHACRYLATE; RESOLUTION LIMITS; BEAM LITHOGRAPHY; ELECTRON RESIST; PMMA; IRRADIATION; EXPOSURE; DEPOLYMERIZATION AB The sensitivity of various polymers to radiation damage by soft X-rays has been measured previously with scanning transmission X-ray microscopes. However, the critical dose values reported by different groups for the same material differ by more than 100%. Possible sources of this variability are investigated here for poly(methyl methacrylate) (PMMA) using controlled exposure to monochromatic soft X-rays at 300 eV. Radiation sensitivity, judged by several different criteria, was evaluated as a function of dose rate, pre-exposure thermal treatments and X-ray polarization. Both the measured critical dose and the dose required to initiate negative mode (cross-linking) were observed to depend only on dose, not the other factors explored. A method of determining detector efficiency from the dose required to initiate negative mode in PMMA is outlined. This method was applied to many of the soft X-ray STXMs presently operating to derive the efficiencies of their transmitted X-ray detectors in the C 1s absorption-edge region. C1 [Leontowich, Adam F. G.; Hitchcock, Adam P.] McMaster Univ, Brockhouse Inst Mat Res, Hamilton, ON L8S 4M1, Canada. [Tyliszczak, Tolek] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Weigand, Markus] Max Planck Inst Intelligent Syst, D-70569 Stuttgart, Baden Wurttembe, Germany. [Wang, Jian; Karunakaran, Chithra] Canadian Light Source Inc, Saskatoon, SK S7N 0X4, Canada. RP Leontowich, AFG (reprint author), McMaster Univ, Brockhouse Inst Mat Res, 1280 Main St W, Hamilton, ON L8S 4M1, Canada. EM leontoaf@mcmaster.ca RI Wang, Jian/M-1805-2013 FU Natural Sciences and Engineering Research Council (NSERC, Canada); Canadian Foundation for Innovation (CFI); Canada Research Chairs program; Office of Energy Research, Office of Basic Energy Sciences, Materials Sciences Division of the US Department of Energy [DE-AC02-05CH11231]; NSERC; CIHR; NRC; University of Saskatchewan; German Minister fur Bildung und Forschung (BMBF) [05 KS4We1/6]; ALS; CLS FX This research was supported by the Natural Sciences and Engineering Research Council (NSERC, Canada), the Canadian Foundation for Innovation (CFI) and the Canada Research Chairs program. We thank all the staff scientists at the various facilities for their expert support and assistance, including Benjamin Watts and Jorg Raabe (SLS), Yingshen Lu and James Dynes (CLS), and David Kilcoyne (ALS). Frank Gibbs is thanked for performing the TGA measurement. The ALS is supported by the Director, Office of Energy Research, Office of Basic Energy Sciences, Materials Sciences Division of the US Department of Energy, under Contract No. DE-AC02-05CH11231. The CLS is supported by NSERC, CIHR, NRC and the University of Saskatchewan. The PolLux end-station was financed by the German Minister fur Bildung und Forschung (BMBF), contract 05 KS4We1/6. This report contains data created at the MAXYMUS STXM of the Department Schutz, MPI-IS Stuttgart at BESSY II, Berlin. AFGL acknowledges support from an ALS doctoral fellowship in residence and the CLS graduate student travel support program. NR 66 TC 11 Z9 11 U1 3 U2 13 PU INT UNION CRYSTALLOGRAPHY PI CHESTER PA 2 ABBEY SQ, CHESTER, CH1 2HU, ENGLAND SN 1600-5775 J9 J SYNCHROTRON RADIAT JI J. Synchrot. Radiat. PD NOV PY 2012 VL 19 BP 976 EP 987 DI 10.1107/S0909049512034486 PN 6 PG 12 WC Instruments & Instrumentation; Optics; Physics, Applied SC Instruments & Instrumentation; Optics; Physics GA 024ZL UT WOS:000310151000018 PM 23093758 ER PT J AU Holton, JM Nielsen, C Frankel, KA AF Holton, James M. Nielsen, Chris Frankel, Kenneth A. TI The point-spread function of fiber-coupled area detectors SO JOURNAL OF SYNCHROTRON RADIATION LA English DT Article; Proceedings Paper CT International Workshop on Improving Data Qualityand Quantity for XAFS Experiments CY APR 12-13, 2011 CL Tsukuba, JAPAN DE protein crystallography X-ray detector; CCD; phosphor; fiber optic ID SCATTERING FACTORS; DIFFRACTION DATA; CRYSTALLOGRAPHY AB The point-spread function (PSF) of a fiber-optic taper-coupled CCD area detector was measured over five decades of intensity using a 20 mu m X-ray beam and similar to 2000-fold averaging. The 'tails' of the PSF clearly revealed that it is neither Gaussian nor Lorentzian, but instead resembles the solid angle subtended by a pixel at a point source of light held a small distance (similar to 27 mu m) above the pixel plane. This converges to an inverse cube law far from the beam impact point. Further analysis revealed that the tails are dominated by the fiber-optic taper, with negligible contribution from the phosphor, suggesting that the PSF of all fiber-coupled CCD-type detectors is best described as a Moffat function. C1 [Holton, James M.] Univ Calif San Francisco, Dept Biochem & Biophys, San Francisco, CA 94158 USA. [Holton, James M.; Frankel, Kenneth A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Nielsen, Chris] Area Detector Syst Corp, Poway, CA 92064 USA. RP Holton, JM (reprint author), Univ Calif San Francisco, Dept Biochem & Biophys, San Francisco, CA 94158 USA. EM jmholton@lbl.gov FU National Institutes of Health [GM073210, GM082250, GM094625]; Integrated Diffraction Analysis Technologies (IDAT) program [DE-AC02-05CH11231]; US Department of Energy at Lawrence Berkeley National Laboratory FX We would like to thank Gerd Rosenbaum, Robert Fischetti, Roger Durst, Sol Gruner and Michael Blum for extremely helpful discussions of this manuscript. This work was supported by grants from the National Institutes of Health (GM073210, GM082250 and GM094625) and the Integrated Diffraction Analysis Technologies (IDAT) program under Contract Number DE-AC02-05CH11231 with the US Department of Energy at Lawrence Berkeley National Laboratory. NR 21 TC 6 Z9 6 U1 2 U2 12 PU INT UNION CRYSTALLOGRAPHY PI CHESTER PA 2 ABBEY SQ, CHESTER, CH1 2HU, ENGLAND SN 1600-5775 J9 J SYNCHROTRON RADIAT JI J. Synchrot. Radiat. PD NOV PY 2012 VL 19 BP 1006 EP 1011 DI 10.1107/S0909049512035571 PN 6 PG 6 WC Instruments & Instrumentation; Optics; Physics, Applied SC Instruments & Instrumentation; Optics; Physics GA 024ZL UT WOS:000310151000022 PM 23093762 ER PT J AU Qin, ZY Lai, B Landero, J Caruso, JA AF Qin, Zhenyu Lai, Barry Landero, Julio Caruso, Joseph A. TI Coupling transmission electron microscopy with synchrotron radiation X-ray fluorescence microscopy to image vascular copper SO JOURNAL OF SYNCHROTRON RADIATION LA English DT Article; Proceedings Paper CT International Workshop on Improving Data Qualityand Quantity for XAFS Experiments CY APR 12-13, 2011 CL Tsukuba, JAPAN DE transmission electron microscopy; synchrotron radiation X-ray fluorescence microscopy; copper; imaging; macrophage; aorta ID PLASMA-MASS SPECTROMETRY; ESSENTIAL-HYPERTENSION; LYSYL OXIDASE; CELLS; REVEALS; MICE; ZINC; DISEASE; WILSON; SERUM AB Recently, using synchrotron radiation X-ray fluorescence microscopy (SRXRF), the copper accumulation in rat aortic elastin and copper topography in human THP-1 cell monolayer have been described. However, it is necessary to locate more accurately cellular copper in the vascular cells and tissues. In the current study, SRXRF coupling with transmission electron microscopy (TEM) was used to image copper in sections of human THP-1 cells and mouse aorta. The results showed that sections of 1 mu m thickness are required for SRXRF producing a correlative image with TEM between copper topography and cellular ultrastructure. As compared with SRXRF alone, coupling TEM with SRXRF can clearly identify the location of copper in the nucleus and nucleolus in nondividing THP-1 cell sections, and can differentiate the copper location at elastic laminae from collagen in mouse aortic sections. Thus, these results revealed new information about the copper topography in vascular cells and tissues and highlighted the potential of TEM-SRXRF to investigate the role of copper in macrophage and aortic homeostasis. C1 [Qin, Zhenyu] Univ Texas Hlth Sci Ctr San Antonio, Dept Surg, Div Vasc Surg, San Antonio, TX 78229 USA. [Qin, Zhenyu] Univ Cincinnati, Dept Med, Div Cardiovasc Dis, Cincinnati, OH 45267 USA. [Lai, Barry] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. [Landero, Julio; Caruso, Joseph A.] Univ Cincinnati, Dept Chem, Cincinnati, OH 45267 USA. RP Qin, ZY (reprint author), Univ Texas Hlth Sci Ctr San Antonio, Dept Surg, Div Vasc Surg, San Antonio, TX 78229 USA. EM qinz@uthscsa.edu FU AHA National Scientist Development Grant [0835268N]; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work was supported by an AHA National Scientist Development Grant (0835268N). Use of the Advanced Photon Source was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 45 TC 5 Z9 5 U1 1 U2 9 PU INT UNION CRYSTALLOGRAPHY PI CHESTER PA 2 ABBEY SQ, CHESTER, CH1 2HU, ENGLAND SN 1600-5775 J9 J SYNCHROTRON RADIAT JI J. Synchrot. Radiat. PD NOV PY 2012 VL 19 BP 1043 EP 1049 DI 10.1107/S090904951203405X PN 6 PG 7 WC Instruments & Instrumentation; Optics; Physics, Applied SC Instruments & Instrumentation; Optics; Physics GA 024ZL UT WOS:000310151000028 PM 23093768 ER PT J AU Winarski, RP Holt, MV Rose, V Fuesz, P Carbaugh, D Benson, C Shu, DM Kline, D Stephenson, GB McNulty, I Maser, J AF Winarski, Robert P. Holt, Martin V. Rose, Volker Fuesz, Peter Carbaugh, Dean Benson, Christa Shu, Deming Kline, David Stephenson, G. Brian McNulty, Ian Maser, Joerg TI A hard X-ray nanoprobe beamline for nanoscale microscopy SO JOURNAL OF SYNCHROTRON RADIATION LA English DT Article; Proceedings Paper CT International Workshop on Improving Data Qualityand Quantity for XAFS Experiments CY APR 12-13, 2011 CL Tsukuba, JAPAN DE X-ray nanoprobe; X-ray microscopy; zone plate; X-ray fluorescence; nanodiffraction; nanotomography ID ADVANCED-PHOTON-SOURCE; ZONE PLATES; CONTRAST AB The Hard X-ray Nanoprobe Beamline (or Nanoprobe Beamline) is an X-ray microscopy facility incorporating diffraction, fluorescence and full-field imaging capabilities designed and operated by the Center for Nanoscale Materials and the Advanced Photon Source at Sector 26 of the Advanced Photon Source at Argonne National Laboratory. This facility was constructed to probe the nanoscale structure of biological, environmental and material sciences samples. The beamline provides intense focused X-rays to the Hard X-ray Nanoprobe (or Nanoprobe) which incorporates Fresnel zone plate optics and a precision laser sensing and control system. The beamline operates over X-ray energies from 3 to 30 keV, enabling studies of most elements in the periodic table, with a particular emphasis on imaging transition metals. C1 [Winarski, Robert P.; Holt, Martin V.; Rose, Volker; Carbaugh, Dean; McNulty, Ian; Maser, Joerg] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60441 USA. [Rose, Volker; Fuesz, Peter; Benson, Christa; Shu, Deming; Kline, David; Stephenson, G. Brian; Maser, Joerg] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60441 USA. RP Winarski, RP (reprint author), Argonne Natl Lab, Ctr Nanoscale Mat, 9700 S Cass Ave, Argonne, IL 60441 USA. EM winarski@anl.gov RI Maser, Jorg/K-6817-2013; Rose, Volker/B-1103-2008 OI Rose, Volker/0000-0002-9027-1052 FU US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX Use of the Center for Nanoscale Materials and the Advanced Photon Source was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under contract No. DE-AC02-06CH11357. NR 34 TC 55 Z9 55 U1 2 U2 59 PU INT UNION CRYSTALLOGRAPHY PI CHESTER PA 2 ABBEY SQ, CHESTER, CH1 2HU, ENGLAND SN 1600-5775 J9 J SYNCHROTRON RADIAT JI J. Synchrot. Radiat. PD NOV PY 2012 VL 19 BP 1056 EP 1060 DI 10.1107/S0909049512036783 PN 6 PG 5 WC Instruments & Instrumentation; Optics; Physics, Applied SC Instruments & Instrumentation; Optics; Physics GA 024ZL UT WOS:000310151000030 PM 23093770 ER PT J AU Reid, BA Samushia, L White, M Percival, WJ Manera, M Padmanabhan, N Ross, AJ Sanchez, AG Bailey, S Bizyaev, D Bolton, AS Brewington, H Brinkmann, J Brownstein, JR Cuesta, AJ Eisenstein, DJ Gunn, JE Honscheid, K Malanushenko, E Malanushenko, V Maraston, C McBride, CK Muna, D Nichol, RC Oravetz, D Pan, K de Putter, R Roe, NA Ross, NP Schlegel, DJ Schneider, DP Seo, HJ Shelden, A Sheldon, ES Simmons, A Skibba, RA Snedden, S Swanson, MEC Thomas, D Tinker, J Tojeiro, R Verde, L Wake, DA Weaver, BA Weinberg, DH Zehavi, I Zhao, GB AF Reid, Beth A. Samushia, Lado White, Martin Percival, Will J. Manera, Marc Padmanabhan, Nikhil Ross, Ashley J. Sanchez, Ariel G. Bailey, Stephen Bizyaev, Dmitry Bolton, Adam S. Brewington, Howard Brinkmann, J. Brownstein, Joel R. Cuesta, Antonio J. Eisenstein, Daniel J. Gunn, James E. Honscheid, Klaus Malanushenko, Elena Malanushenko, Viktor Maraston, Claudia McBride, Cameron K. Muna, Demitri Nichol, Robert C. Oravetz, Daniel Pan, Kaike de Putter, Roland Roe, N. A. Ross, Nicholas P. Schlegel, David J. Schneider, Donald P. Seo, Hee-Jong Shelden, Alaina Sheldon, Erin S. Simmons, Audrey Skibba, Ramin A. Snedden, Stephanie Swanson, Molly E. C. Thomas, Daniel Tinker, Jeremy Tojeiro, Rita Verde, Licia Wake, David A. Weaver, Benjamin A. Weinberg, David H. Zehavi, Idit Zhao, Gong-Bo TI The clustering of galaxies in the SDSS-III Baryon Oscillation Spectroscopic Survey: measurements of the growth of structure and expansion rate at z=0.57 from anisotropic clustering SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Review DE galaxies: haloes; galaxies: statistics; cosmological parameters; large-scale structure of Universe ID DIGITAL SKY SURVEY; LUMINOUS RED GALAXIES; DARK ENERGY SURVEY; 2-POINT CORRELATION-FUNCTION; HUBBLE-SPACE-TELESCOPE; REDSHIFT SURVEY; ACOUSTIC-OSCILLATIONS; COSMOLOGICAL CONSTANT; POWER-SPECTRUM; LINEAR REGIME AB We analyse the anisotropic clustering of massive galaxies from the Sloan Digital Sky Survey III Baryon Oscillation Spectroscopic Survey (BOSS) Data Release 9 (DR9) sample, which consists of 264-283 galaxies in the redshift range 0.43 < z < 0.7 spanning 3275 deg(2). Both peculiar velocities and errors in the assumed redshiftdistance relation (AlcockPaczynski effect) generate correlations between clustering amplitude and orientation with respect to the line of sight. Together with the sharp baryon acoustic oscillation (BAO) standard ruler, our measurements of the broad-band shape of the monopole and quadrupole correlation functions simultaneously constrain the comoving angular diameter distance (2190 +/- 61 Mpc) to z = 0.57, the Hubble expansion rate at z = 0.57 (92.4 +/- 4.5 km s(-1) Mpc(-1)) and the growth rate of structure at that same redshift (d(sigma 8)/d ln a = 0.43 +/- 0.069). Our analysis provides the best current direct determination of both DA and H in galaxy clustering data using this technique. If we further assume a cold dark matter expansion history, our growth constraint tightens to d(sigma 8)/d ln a = 0.415 +/- 0.034. In combination with the cosmic microwave background, our measurements of D-A,H and d(sigma 8)/d ln a all separately require dark energy at z > 0.57, and when combined imply Omega(A) = 0.74 +/- 0.016, independent of the Universe's evolution at z < 0.57. All of these constraints assume scale-independent linear growth, and assume general relativity to compute both O(10 per cent) non-linear model corrections and our errors. In our companion paper, Samushia et al., we explore further cosmological implications of these observations. C1 [Reid, Beth A.; White, Martin; Bailey, Stephen; Roe, N. A.; Ross, Nicholas P.; Schlegel, David J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Samushia, Lado; Percival, Will J.; Manera, Marc; Ross, Ashley J.; Maraston, Claudia; Nichol, Robert C.; Thomas, Daniel; Tojeiro, Rita; Zhao, Gong-Bo] Univ Portsmouth, Inst Cosmol & Gravitat, Portsmouth P01 3FX, Hants, England. [Samushia, Lado] Ilia State Univ, Natl Abastumani Astrophys Observ, GE-1060 Tbilisi, Rep of Georgia. [White, Martin] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [White, Martin] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. [Padmanabhan, Nikhil; Cuesta, Antonio J.] Yale Univ, Dept Phys, New Haven, CT 06520 USA. [Sanchez, Ariel G.] Max Planck Inst Extraterr Phys, D-85741 Garching, Germany. [Bizyaev, Dmitry; Brewington, Howard; Brinkmann, J.; Malanushenko, Elena; Malanushenko, Viktor; Oravetz, Daniel; Pan, Kaike; Shelden, Alaina; Simmons, Audrey; Snedden, Stephanie] Apache Point Observ, Sunspot, NM 88349 USA. [Bolton, Adam S.; Brownstein, Joel R.] Univ Utah, Dept Phys & Astron, Salt Lake City, UT 84112 USA. [Eisenstein, Daniel J.; McBride, Cameron K.; Swanson, Molly E. C.] Harvard Smithsonian Ctr Astrophys, Cambridge, MA 02138 USA. [Gunn, James E.] Princeton Univ, Dept Astrophys Sci, Princeton, NJ 08544 USA. [Honscheid, Klaus; Weinberg, David H.] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. [Honscheid, Klaus; Weinberg, David H.] Ohio State Univ, CCAPP, Columbus, OH 43210 USA. [Muna, Demitri; Tinker, Jeremy; Weaver, Benjamin A.] NYU, Ctr Cosmol & Particle Phys, New York, NY 10003 USA. [de Putter, Roland] Univ Valencia, CSIC, Inst Fis Corpuscular, Valencia 46701, Spain. [de Putter, Roland; Verde, Licia] Univ Barcelona, IEEC UB, ICC, E-08028 Barcelona, Spain. [Schneider, Donald P.] Penn State Univ, Dept Astron & Astrophys, University Pk, PA 16802 USA. [Schneider, Donald P.] Penn State Univ, Inst Gravitat & Cosmos, University Pk, PA 16802 USA. [Seo, Hee-Jong] Univ Calif Berkeley, LBL, Berkeley Ctr Cosmol Phys, Berkeley, CA 94720 USA. [Seo, Hee-Jong] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Sheldon, Erin S.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Skibba, Ramin A.] Univ Arizona, Steward Observ, Tucson, AZ 85721 USA. [Verde, Licia] Passeig Lluis Co 23, ICREA, Barcelona 08010, Spain. [Wake, David A.] Yale Univ, Yale Ctr Astron & Astrophys, New Haven, CT 06520 USA. [Zehavi, Idit] Case Western Reserve Univ, Dept Astron, Cleveland, OH 44106 USA. [Zhao, Gong-Bo] Chinese Acad Sci, Natl Astron Observ, Beijing 100012, Peoples R China. RP Reid, BA (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM beth.ann.reid@gmail.com RI White, Martin/I-3880-2015; OI White, Martin/0000-0001-9912-5070; Cuesta Vazquez, Antonio Jose/0000-0002-4153-9470; Verde, Licia/0000-0003-2601-8770 NR 107 TC 187 Z9 188 U1 2 U2 17 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD NOV PY 2012 VL 426 IS 4 BP 2719 EP 2737 DI 10.1111/j.1365-2966.2012.21779.x PG 19 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 023VI UT WOS:000310064400008 ER PT J AU Mateos, S Alonso-Herrero, A Carrera, FJ Blain, A Watson, MG Barcons, X Braito, V Severgnini, P Donley, JL Stern, D AF Mateos, S. Alonso-Herrero, A. Carrera, F. J. Blain, A. Watson, M. G. Barcons, X. Braito, V. Severgnini, P. Donley, J. L. Stern, D. TI Using the Bright Ultrahard XMM-Newton survey to define an IR selection of luminous AGN based on WISE colours SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE galaxies: active; quasars: general; infrared: galaxies ID ACTIVE GALACTIC NUCLEI; SPITZER-SPACE-TELESCOPE; DEEP FIELD-SOUTH; SPECTRAL ENERGY-DISTRIBUTIONS; SWIFT-BAT SURVEY; BLACK-HOLES; MIDINFRARED SELECTION; GALAXIES; QUASARS; SAMPLE AB We present a highly complete and reliable mid-infrared (MIR) colour selection of luminous active galactic nucleus (AGN) candidates using the 3.4, 4.6 and 12 mu m bands of the Wide-field Infrared Survey Explorer (WISE) survey. The MIR colour wedge was defined using the wide-angle Bright Ultrahard XMMNewton survey (BUXS), one of the largest complete flux-limited samples of bright (f4.5--10 keV >6x10-14 erg s-1 cm -2) ultrahard (4.510? keV) X-ray-selected AGN to date. The BUXS includes 258 objects detected over a total sky area of 44.43?deg2 of which 251 are spectroscopically identified and classified, with 145 being type 1 AGN and 106 type 2 AGN. Our technique is designed to select objects with red MIR power-law spectral energy distributions (SEDs) in the three shortest bands of WISE and properly accounts for the errors in the photometry and deviations of the MIR SEDs from a pure power-law. The completeness of the MIR selection is a strong function of luminosity. At L210?keV >1044 ? erg?s-1, where the AGN is expected to dominate the MIR emission, 97.1-4.8+2.2 and 76.5-18.4+13.3 per cent of the BUXS type 1 and type 2 AGN, respectively, meet the selection. Our technique shows one of the highest reliability and efficiency of detection of the X-ray-selected luminous AGN population with WISE amongst those in the literature. In the area covered by BUXS our selection identifies 2755 AGN candidates detected with signal-to-noise ratio =5 in the three shorter wavelength bands of WISE with 38.5 per cent having a detection at 210?keV X-ray energies. We also analysed the possibility of including the 22? mu m WISE band to select AGN candidates, but neither the completeness nor the reliability of the selection improves. This is likely due to both the significantly shallower depth at 22 mu m compared with the first three bands of WISE and star formation contributing to the 22 mu m emission at the WISE 22 mu m sensitivity. C1 [Mateos, S.; Alonso-Herrero, A.; Carrera, F. J.; Barcons, X.] Univ Cantabria, Inst Fis Cantabria, CSIC, E-39005 Santander, Spain. [Mateos, S.; Blain, A.; Watson, M. G.] Univ Leicester, Leicester LE1 7RH, Leics, England. [Braito, V.] Osserv Astron Brera, Ist Nazl Astrofis, I-23807 Merate, LC, Italy. [Severgnini, P.] INAF Osservatorio Astron Brera, I-20121 Milan, Italy. [Donley, J. L.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Stern, D.] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. RP Mateos, S (reprint author), Univ Cantabria, Inst Fis Cantabria, CSIC, E-39005 Santander, Spain. EM mateos@ifca.unican.es RI Barcons, Xavier/L-3335-2014; Mateos, Silvia/F-9524-2016; Alonso-Herrero, Almudena/H-1426-2015; OI Barcons, Xavier/0000-0003-1081-8861; Mateos, Silvia/0000-0002-1375-2389; Alonso-Herrero, Almudena/0000-0001-6794-2519; Severgnini, Paola/0000-0001-5619-5896; Braito, Valentina/0000-0002-2629-4989 FU NASA; Alfred P. Sloan Foundation; National Science Foundation; U.S. Department of Energy; National Aeronautics and Space Administration; Japanese Monbukagakusho; Max Planck Society; Higher Education Funding Council for England; European Organisation for Astronomical Research in the Southern hemisphere, Chile [084.A-0828, 086.A-0612, 087.A-0447]; Spanish Ministry of Economy and Competitiveness [AYA2010-21490-C02-01]; Universidad de Cantabria through the Augusto G. Linares program; Royal Society Wolfson Research Merit Award; LANL Director's Fellowship; ASI [I/009/10/0] FX This work is based on observations obtained with XMM-Newton, an ESA science mission with instruments and contributions directly funded by ESA Member States and NASA. It is also based on data from the Wide-field Infrared Survey Explorer, which is a joint project of the University of California, Los Angeles and the Jet Propulsion Laboratory/California Institute of Technology, funded by the National Aeronautics and Space Administration. Funding for the SDSS and SDSS-II has been provided by the Alfred P. Sloan Foundation, the Participating Institutions, the National Science Foundation, the U.S. Department of Energy, the National Aeronautics and Space Administration, the Japanese Monbukagakusho, the Max Planck Society and the Higher Education Funding Council for England. The SDSS website is http://www.sdss.org/. This work is based on observations collected at the European Organisation for Astronomical Research in the Southern hemisphere, Chile, programme IDs 084.A-0828, 086.A-0612, 087.A-0447. It is also based on observations made with the William Herschel Telescope - operated by the Isaac Newton Group, the Telescopio Nazionale Galileo - operated by the Centro Galileo Galilei and the Gran Telescopio de Canarias installed in the Spanish Observatorio del Roque de los Muchachos of the Instituto de Astrofsica de Canarias, in the island of La Palma. SM, FJC and XB acknowledge financial support by the Spanish Ministry of Economy and Competitiveness through grant AYA2010-21490-C02-01. AAH acknowledges support from the Universidad de Cantabria through the Augusto G. Linares program. AB acknowledges a Royal Society Wolfson Research Merit Award. JLD acknowledges support from the LANL Director's Fellowship. PS acknowledges financial support from ASI (grant No. I/009/10/0). The authors wish to thank the anonymous referee for constructive comments. NR 50 TC 79 Z9 79 U1 0 U2 6 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0035-8711 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD NOV PY 2012 VL 426 IS 4 BP 3271 EP 3281 DI 10.1111/j.1365-2966.2012.21843.x PG 11 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA 023VI UT WOS:000310064400047 ER PT J AU Slavov, GT DiFazio, SP Martin, J Schackwitz, W Muchero, W Rodgers-Melnick, E Lipphardt, MF Pennacchio, CP Hellsten, U Pennacchio, LA Gunter, LE Ranjan, P Vining, K Pomraning, KR Wilhelm, LJ Pellegrini, M Mockler, TC Freitag, M Geraldes, A El-Kassaby, YA Mansfield, SD Cronk, QCB Douglas, CJ Strauss, SH Rokhsar, D Tuskan, GA AF Slavov, Gancho T. DiFazio, Stephen P. Martin, Joel Schackwitz, Wendy Muchero, Wellington Rodgers-Melnick, Eli Lipphardt, Mindie F. Pennacchio, Christa P. Hellsten, Uffe Pennacchio, Len A. Gunter, Lee E. Ranjan, Priya Vining, Kelly Pomraning, Kyle R. Wilhelm, Larry J. Pellegrini, Matteo Mockler, Todd C. Freitag, Michael Geraldes, Armando El-Kassaby, Yousry A. Mansfield, Shawn D. Cronk, Quentin C. B. Douglas, Carl J. Strauss, Steven H. Rokhsar, Dan Tuskan, Gerald A. TI Genome resequencing reveals multiscale geographic structure and extensive linkage disequilibrium in the forest tree Populus trichocarpa SO NEW PHYTOLOGIST LA English DT Article DE allele frequency gradients; black cottonwood (Populus trichocarpa); genome resequencing; linkage disequilibrium (LD); population structure; recombination ID NUCLEOTIDE DIVERSITY; POPULATION-STRUCTURE; GENETIC-VARIATION; BLACK COTTONWOOD; ARABIDOPSIS-THALIANA; RECOMBINATION RATES; MULTILOCUS PATTERNS; DEMOGRAPHIC HISTORY; PACIFIC-NORTHWEST; WIDE ASSOCIATION AB Plant population genomics informs evolutionary biology, breeding, conservation and bioenergy feedstock development. For example, the detection of reliable phenotypegenotype associations and molecular signatures of selection requires a detailed knowledge about genome-wide patterns of allele frequency variation, linkage disequilibrium and recombination. We resequenced 16 genomes of the model tree Populus trichocarpa and genotyped 120 trees from 10 subpopulations using 29 213 single-nucleotide polymorphisms. Significant geographic differentiation was present at multiple spatial scales, and range-wide latitudinal allele frequency gradients were strikingly common across the genome. The decay of linkage disequilibrium with physical distance was slower than expected from previous studies in Populus, with r(2) dropping below 0.2 within 36 kb. Consistent with this, estimates of recent effective population size from linkage disequilibrium (N-e approximate to 4000-6000) were remarkably low relative to the large census sizes of P. trichocarpa stands. Fine-scale rates of recombination varied widely across the genome, but were largely predictable on the basis of DNA sequence and methylation features. Our results suggest that genetic drift has played a significant role in the recent evolutionary history of P. trichocarpa. Most importantly, the extensive linkage disequilibrium detected suggests that genome-wide association studies and genomic selection in undomesticated populations may be more feasible in Populus than previously assumed. C1 [Slavov, Gancho T.; DiFazio, Stephen P.; Rodgers-Melnick, Eli; Lipphardt, Mindie F.] W Virginia Univ, Dept Biol, Morgantown, WV 26506 USA. [Slavov, Gancho T.] Aberystwyth Univ, Inst Biol Environm & Rural Sci, Aberystwyth SY23 3EB, Dyfed, Wales. [Martin, Joel; Schackwitz, Wendy; Pennacchio, Christa P.; Hellsten, Uffe; Pennacchio, Len A.; Rokhsar, Dan] US DOE, Joint Genome Inst, Walnut Creek, CA 94598 USA. [Muchero, Wellington; Gunter, Lee E.; Ranjan, Priya; Tuskan, Gerald A.] Oak Ridge Natl Lab, BioSci Div, Oak Ridge, TN 37831 USA. [Vining, Kelly; Strauss, Steven H.] Oregon State Univ, Dept Forest Ecosyst & Soc, Corvallis, OR 97331 USA. [Pomraning, Kyle R.; Freitag, Michael] Oregon State Univ, Dept Biochem & Biophys, Corvallis, OR 97331 USA. [Wilhelm, Larry J.] Oregon Hlth & Sci Univ, Beaverton, OR 97006 USA. [Pellegrini, Matteo] Univ Calif Los Angeles, Dept Mol Cell & Dev Biol, Los Angeles, CA 90095 USA. [Mockler, Todd C.] Donald Danforth Plant Sci Ctr, St Louis, MO 63132 USA. [Geraldes, Armando; Cronk, Quentin C. B.; Douglas, Carl J.] Univ British Columbia, Dept Bot, Vancouver, BC V6T 1Z4, Canada. [El-Kassaby, Yousry A.] Univ British Columbia, Dept Forest Sci, Vancouver, BC V6T 1Z4, Canada. [Mansfield, Shawn D.] Univ British Columbia, Dept Wood Sci, Vancouver, BC V6T 1Z4, Canada. RP Slavov, GT (reprint author), W Virginia Univ, Dept Biol, Morgantown, WV 26506 USA. EM gts@aber.ac.uk RI Douglas, Carl/B-1384-2013; Mockler, Todd/L-2609-2013; El-Kassaby, Yousry/K-9856-2016; Gunter, Lee/L-3480-2016; Tuskan, Gerald/A-6225-2011; OI Mockler, Todd/0000-0002-0462-5775; El-Kassaby, Yousry/0000-0002-4887-8977; Gunter, Lee/0000-0003-1211-7532; Tuskan, Gerald/0000-0003-0106-1289; Pomraning, Kyle/0000-0003-2324-2881; muchero, wellington/0000-0002-0200-9856; Cronk, Quentin/0000-0002-4027-7368 FU BioEnergy Science Center, a US Department of Energy (DOE) Bioenergy Research Center (Office of Biological and Environmental Research in the DOE Office of Science); Province of British Columbia through Genome British Columbia Applied Genomics Innovation Program [103BIO]; Office of Science of the DOE [DE-AC02-05CH11231] FX Funding was provided by the BioEnergy Science Center, a US Department of Energy (DOE) Bioenergy Research Center (Office of Biological and Environmental Research in the DOE Office of Science) and by the Province of British Columbia through Genome British Columbia Applied Genomics Innovation Program project 103BIO. The work conducted by the DOE Joint Genome Institute was supported by the Office of Science of the DOE under Contract No. DE-AC02-05CH11231. Reinhard Stettler, Jon Johnson, Brian Stanton, Richard Shuren, Nancy Engle, Xiaohan Yang and Stan Wullschleger provided assistance with the collection of plant materials. We thank Reinhard Stettler, Glenn Howe, the New Phytologist Editor and three anonymous reviewers for their comments on earlier versions of the manuscript. NR 69 TC 71 Z9 73 U1 7 U2 112 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0028-646X J9 NEW PHYTOL JI New Phytol. PD NOV PY 2012 VL 196 IS 3 BP 713 EP 725 DI 10.1111/j.1469-8137.2012.04258.x PG 13 WC Plant Sciences SC Plant Sciences GA 019RO UT WOS:000309757200011 PM 22861491 ER PT J AU Karve, AA Jawdy, SS Gunter, LE Allen, SM Yang, XH Tuskan, GA Wullschleger, SD Weston, DJ AF Karve, Abhijit A. Jawdy, Sara S. Gunter, Lee E. Allen, Sara M. Yang, Xiaohan Tuskan, Gerald A. Wullschleger, Stan D. Weston, David J. TI Initial characterization of shade avoidance response suggests functional diversity between Populus phytochrome B genes SO NEW PHYTOLOGIST LA English DT Article DE Arabidopsis; far-red; phytochrome; Populus; RNA-seq; shade ID ARABIDOPSIS-THALIANA L; PHYSIOLOGICAL-RESPONSES; PETIOLE ELONGATION; NEGATIVE REGULATOR; PLANT PHYTOCHROMES; BLACK COTTONWOOD; FLOWERING TIME; LIGHT SIGNALS; MUTANT LACKS; EXPRESSION AB Shade avoidance signaling involves perception of incident red/far-red (R/FR) light by phytochromes (PHYs) and modulation of downstream transcriptional networks. Although these responses are well studied in Arabidopsis, little is known about the role of PHYs and the transcriptional responses to shade in the woody perennial Populus. Tissue expression and subcellular localization of Populus PHYs was studied by quantitative real-time PCR (qRT-PCR) and protoplast transient assay. Transgenic lines with altered PHYB1 and/or PHYB2 expression were used in phenotypic assays and transcript profiling with qRT-PCR. RNA-Seq was used to identify transcriptional responses to enriched FR light. All three PHYs were differentially expressed among tissue types and PHYBs were targeted to the nucleus under white light. Populus PHYB1 rescued Arabidopsis phyB mutant phenotypes. Phenotypes of Populus transgenic lines and the expression of candidate shade response genes suggested that PHYB1 and PHYB2 have distinct yet overlapping functions. RNA-Seq analysis indicated that genes associated with cell wall modification and brassinosteroid signaling were induced under enriched FR light in Populus. This study is an initial attempt at deciphering the role of Populus PHYs by evaluating transcriptional reprogramming to enriched FR and demonstrates functional diversity and overlap of the Populus PHYB1 and PHYB2 in regulating shade responses. C1 [Allen, Sara M.] Univ Tennessee, Dept Plant Sci, Knoxville, TN USA. [Wullschleger, Stan D.] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. [Karve, Abhijit A.; Jawdy, Sara S.; Gunter, Lee E.; Allen, Sara M.; Yang, Xiaohan; Tuskan, Gerald A.; Weston, David J.] Oak Ridge Natl Lab, BioSci Div, Oak Ridge, TN 37831 USA. RP Karve, AA (reprint author), Brookhaven Natl Lab, Dept Med, Upton, NY 11973 USA. EM akarve@g.clemson.edu RI Gunter, Lee/L-3480-2016; Wullschleger, Stan/B-8297-2012; Tuskan, Gerald/A-6225-2011; Yang, Xiaohan/A-6975-2011 OI Gunter, Lee/0000-0003-1211-7532; Wullschleger, Stan/0000-0002-9869-0446; Tuskan, Gerald/0000-0003-0106-1289; Yang, Xiaohan/0000-0001-5207-4210 FU Genomic Science Program, US Department of Energy, Office of Science, Biological and Environmental Research, as part of the Plant-Microbe Interfaces Scientific Focus Area; US Department of Energy [DE-AC05-00OR22725] FX This research was sponsored by the Genomic Science Program, US Department of Energy, Office of Science, Biological and Environmental Research, as part of the Plant-Microbe Interfaces Scientific Focus Area (http://pmi.ornl.gov). Oak Ridge National Laboratory is managed by UT-Battelle LLC, for the US Department of Energy under contract DE-AC05-00OR22725. NR 70 TC 2 Z9 2 U1 1 U2 36 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0028-646X EI 1469-8137 J9 NEW PHYTOL JI New Phytol. PD NOV PY 2012 VL 196 IS 3 BP 726 EP 737 DI 10.1111/j.1469-8137.2012.04288.x PG 12 WC Plant Sciences SC Plant Sciences GA 019RO UT WOS:000309757200012 PM 22943289 ER PT J AU Wang, DA Gauld, IC Yoder, GL Ott, LJ Flanagan, GF Francis, MW Popov, EL Carbajo, JJ Jain, PK Wagner, JC Gehin, JC AF Wang, Dean Gauld, Ian C. Yoder, Graydon L. Ott, Larry J. Flanagan, George F. Francis, Matthew W. Popov, Emilian L. Carbajo, Juan J. Jain, Prashant K. Wagner, John C. Gehin, Jess C. TI STUDY OF FUKUSHIMA DAIICHI NUCLEAR POWER STATION UNIT 4 SPENT-FUEL POOL SO NUCLEAR TECHNOLOGY LA English DT Article DE Fukushima Daiichi; spent-fuel pool; evaporation AB A study on the Fukushima Daiichi nuclear power station spent-fuel pool (SFP) at Unit 4 (SFP4) is presented in this paper. We discuss the design characteristics of SFP4 and its decay heat load in detail and provide a model that we developed to estimate the SFP evaporation rate based on the SFP temperature. The SFP level of SFP4 following the March 11, 2011, accident is predicted based on the fundamental conservation laws of mass and energy. Our predicted SFP level and temperatures are in good agreement with measured data and are consistent with Tokyo Electric Power Company evaluation results. C1 [Wang, Dean; Gauld, Ian C.; Yoder, Graydon L.; Ott, Larry J.; Flanagan, George F.; Francis, Matthew W.; Popov, Emilian L.; Carbajo, Juan J.; Jain, Prashant K.; Wagner, John C.; Gehin, Jess C.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Wang, DA (reprint author), Oak Ridge Natl Lab, 1 Bethel Valley Rd 6167, Oak Ridge, TN 37831 USA. EM wangda@ornl.gov RI Wagner, John/K-3644-2015; OI Wagner, John/0000-0003-0257-4502; Gehin, Jess/0000-0001-8337-9551; Gauld, Ian/0000-0002-3893-7515 FU UT-Battelle LLC [DE-AC05-00OR22725]; U.S. Department of Energy FX This manuscript has been authored by UT-Battelle LLC under contract DE-AC05-00OR22725 with the U.S. Department of Energy. NR 5 TC 5 Z9 5 U1 0 U2 13 PU AMER NUCLEAR SOC PI LA GRANGE PK PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA SN 0029-5450 J9 NUCL TECHNOL JI Nucl. Technol. PD NOV PY 2012 VL 180 IS 2 BP 205 EP 215 PG 11 WC Nuclear Science & Technology SC Nuclear Science & Technology GA 018WD UT WOS:000309696600005 ER PT J AU Roecker, C Bowden, NS Carosi, G Heffner, M Jovanovic, I AF Roecker, C. Bowden, N. S. Carosi, G. Heffner, M. Jovanovic, I. TI RECONSTRUCTION ALGORITHMS FOR DIRECTIONAL NEUTRON DETECTION USING A TIME PROJECTION CHAMBER SO NUCLEAR TECHNOLOGY LA English DT Article DE directional neutron detection; neutron imaging; time projection chamber ID FRAMEWORK AB Directional detection of fast neutrons emitted by special nuclear materials can be performed with a time projection chamber. This device permits particle identification and full three-dimensional reconstruction of charged-particle tracks produced by interaction of fast neutrons in the chamber active volume. Single-recoil-proton reconstruction allows rapid pointing, while the reconstruction of two recoil protons produced by a single incident neutron event can enable a measurement with very high angular resolution. Kinematic reconstruction algorithms for both of these cases are presented and their performance assessed using data generated by a simple Monte Carlo simulation and experimental data where those exist. The simulation data are also used to estimate the relative efficiency of both neutron imaging modalities as a function of the volume and pressure of the time projection chamber. C1 [Roecker, C.] Purdue Univ, Sch Nucl Engn, W Lafayette, IN 47907 USA. [Bowden, N. S.; Carosi, G.; Heffner, M.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Jovanovic, I.] Penn State Univ, Dept Mech & Nucl Engn, University Pk, PA 16802 USA. RP Roecker, C (reprint author), Purdue Univ, Sch Nucl Engn, W Lafayette, IN 47907 USA. EM ijovanovic@psu.edu OI Bowden, Nathaniel/0000-0002-6115-0956 FU U.S. Department of Energy, National Nuclear Security Administration, Office of Non-proliferation and Verification Research and Development; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This research is supported by the U.S. Department of Energy, National Nuclear Security Administration, Office of Non-proliferation and Verification Research and Development. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under contract DE-AC52-07NA27344. NR 16 TC 0 Z9 0 U1 0 U2 6 PU AMER NUCLEAR SOC PI LA GRANGE PK PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA SN 0029-5450 J9 NUCL TECHNOL JI Nucl. Technol. PD NOV PY 2012 VL 180 IS 2 BP 231 EP 240 PG 10 WC Nuclear Science & Technology SC Nuclear Science & Technology GA 018WD UT WOS:000309696600007 ER PT J AU Gaathon, O Adam, JD Krishnaswamy, SV Kysar, JW Bakhru, S Bakhru, H Welch, DO Osgood, RM AF Gaathon, O. Adam, J. D. Krishnaswamy, S. V. Kysar, J. W. Bakhru, S. Bakhru, H. Welch, D. O. Osgood, R. M., Jr. TI Planar single-crystal thin-films of YAG obtained by ion implantation and thermal exfoliation: Mechanical properties SO OPTICAL MATERIALS LA English DT Article DE Yttrium Aluminum Garnet; Thin-film; Crystal Ion slicing; Ion implantation ID POTASSIUM TANTALATE FILMS; LITHIUM-NIOBATE; EPITAXIAL LIFTOFF; LINBO3 FILMS; SI AB We report on the fabrication of single-crystal thin films of Yttrium Aluminum Garnet (YAG, Y3Al5O12) obtained by thermal exfoliation from bulk crystals after deep He-ion implantation. The film qualities and exfoliation process were determined by AFM, optical microscopy, SEM, optical profilometer and nanoindentation. The resulting films were subjected to annealing at similar to 1200 degrees C to relax the residual strain and film curvature that arose from the ion implantation process. (C) 2012 Elsevier B.V. All rights reserved. C1 [Gaathon, O.; Kysar, J. W.; Osgood, R. M., Jr.] Columbia Univ, New York, NY 10027 USA. [Adam, J. D.; Krishnaswamy, S. V.] Northrop Grumman Syst Corp, Baltimore, MD 21203 USA. [Bakhru, S.; Bakhru, H.] SUNY Albany, Coll Nanoscale Sci & Engn, Albany, NY 12203 USA. [Welch, D. O.] Brookhaven Natl Lab, Dept Condensed Matter Phys & Mat Sci, Upton, NY 11973 USA. RP Gaathon, O (reprint author), Columbia Univ, New York, NY 10027 USA. EM og2126@columbia.edu FU DARPA ART/CSSA program through The US Army Aviation & Missile Command [W31P4Q-09-C-0528]; US Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886]; NSF [CMMI-0927891]; AFOSR [FA9550-09-1-0048] FX This work was supported by the DARPA ART/CSSA program through The US Army Aviation & Missile Command under Contract No. W31P4Q-09-C-0528. Research was carried out, in part, at the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the US Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. J.W.K. acknowledges support from NSF CMMI-0927891 and AFOSR FA9550-09-1-0048. We would also like to thank Ryan Cooper for his assistance in this work. NR 37 TC 3 Z9 3 U1 4 U2 25 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0925-3467 J9 OPT MATER JI Opt. Mater. PD NOV PY 2012 VL 35 IS 1 BP 25 EP 28 DI 10.1016/j.optmat.2012.06.009 PG 4 WC Materials Science, Multidisciplinary; Optics SC Materials Science; Optics GA 018GO UT WOS:000309648400005 ER PT J AU Seeley, ZM Dai, ZR Kuntz, JD Cherepy, NJ Payne, SA AF Seeley, Z. M. Dai, Z. R. Kuntz, J. D. Cherepy, N. J. Payne, S. A. TI Phase stabilization in transparent Lu2O3:Eu ceramics by lattice expansion SO OPTICAL MATERIALS LA English DT Article DE Transparent ceramic; Lutetium oxide; Gadolinium oxide; Densification; Sinter-HIP ID RARE-EARTH-OXIDES; SCINTILLATORS AB Gadolinium lutetium oxide transparent ceramics doped with europium (Gd,Lu)(2)O-3:Eu were fabricated via vacuum sintering and hot isostatic pressing (HIP). Nano-scale starting powder with the composition GdxLu19-xEu0.1O3 (x = 0, 0.3, 0.6, 0.9, 1.0, and 1.1) were uniaxially pressed and sintered under high vacuum at 1625 degrees C to obtain similar to 97% dense structures with closed porosity. Sintered compacts were then subjected to 200 MPa argon gas at temperatures between 1750 and 1900 degrees C to reach full density. It was observed that a small portion of the Eu3+ ions were exsolved from the Lu2O3 cubic crystal lattice and concentrated at the grain boundaries, where they precipitated into a secondary monoclinic phase creating optical scattering defects. Addition of Gd3+ ions into the Lu2O3 cubic lattice formed the solid solution (Gd,Lu)(2)O-3:Eu and stretched the lattice parameter allowing the larger Eu3+ ions to stay in solid solution, reducing the secondary phase and improving the transparency of the ceramics. Excess gadolinium, however, resulted in a complete phase transformation to monoclinic at pressures and temperatures sufficient for densification. Light yield performance was measured and all samples show equal amounts of the characteristic Eu3+ luminescence, indicating gadolinium addition had no adverse effect. This material has potential to improve the performance of high energy radiography devices. (C) 2012 Elsevier B.V. All rights reserved. C1 [Seeley, Z. M.; Dai, Z. R.; Kuntz, J. D.; Cherepy, N. J.; Payne, S. A.] Lawrence Livermore Natl Lab, Div Chem Sci, Livermore, CA 94550 USA. RP Seeley, ZM (reprint author), Lawrence Livermore Natl Lab, Div Chem Sci, Livermore, CA 94550 USA. EM seeley7@llnl.gov RI Cherepy, Nerine/F-6176-2013 OI Cherepy, Nerine/0000-0001-8561-923X FU U.S. Department of Energy; Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; US DOE, Office of NNSA, Enhanced Surveillance Subprogram [LLNL-JRNL-559892] FX Thanks to Todd Stefanik of Nanocerox Inc., Jeff Roberts for flame spray synthesis, Scott Fisher for mechanical fabrication, Marcia Kellam for optical scatter measurements, and the Confined Large Optical Scintillator Screen and Imaging System (CoLOSSIS) team including Patrick Allen, James Trebes, Daniel Schneberk, and Gary Stone. This work performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344 and funded by the US DOE, Office of NNSA, Enhanced Surveillance Subprogram, LLNL-JRNL-559892. NR 17 TC 8 Z9 9 U1 2 U2 41 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0925-3467 EI 1873-1252 J9 OPT MATER JI Opt. Mater. PD NOV PY 2012 VL 35 IS 1 BP 74 EP 78 DI 10.1016/j.optmat.2012.07.005 PG 5 WC Materials Science, Multidisciplinary; Optics SC Materials Science; Optics GA 018GO UT WOS:000309648400014 ER PT J AU Contreras, MA Mansfield, LM Egaas, B Li, J Romero, M Noufi, R Rudiger-Voigt, E Mannstadt, W AF Contreras, Miguel A. Mansfield, Lorelle M. Egaas, Brian Li, Jian Romero, Manuel Noufi, Rommel Rudiger-Voigt, Eveline Mannstadt, Wolfgang TI Wide bandgap Cu(In,Ga)Se-2 solar cells with improved energy conversion efficiency SO PROGRESS IN PHOTOVOLTAICS LA English DT Article DE CIGS; wide gap; chalcogenides; high efficiency; thin film; high temperature ID THIN-FILMS AB We report on improvements to the energy conversion efficiency of wide bandgap (E-g > 1.2 eV) solar cells on the basis of CuIn1-xGaxSe2. Historically, attaining high efficiency (>16%) from these types of compound semiconductor thin films has been difficult. Nevertheless, by using (a) the alkaline-containing high-temperature EtaMax glass substrates from Schott AG, (b) elevated substrate temperatures of 600-650 degrees C, and (c) high vacuum evaporation from elemental sources following National Renewable Energy Laboratory's three-stage process, we have been able to improve the performance of wider bandgap solar cells with 1.2 < E-g < 1.45 eV. The current densityvoltage (JV) data we present includes efficiencies >18% for absorber bandgaps of similar to 1.30 eV and efficiencies of similar to 16% for bandgaps up to similar to 1.45 eV. In comparing JV parameters in similar materials, we establish gains in the open-circuit voltage and, to a lesser degree, the fill factor value, as the reason for the improved performance. The higher voltages seen in these wide gap materials grown at high substrate temperatures are due to reduced recombination. We establish the existence of random and discrete grains within the CIGS absorbers that yield limited or no generation/collection of minority carriers. We also show that interfacial recombination is the main mechanism limiting additional enhancements to open-circuit voltage and therefore performance. Solar cell results, absorber materials characterization, and experimental details and discussion are presented. Copyright (c) 2012 John Wiley & Sons, Ltd. C1 [Contreras, Miguel A.; Mansfield, Lorelle M.; Egaas, Brian; Li, Jian; Romero, Manuel; Noufi, Rommel] Natl Renewable Energy Lab, Golden, CO USA. [Rudiger-Voigt, Eveline; Mannstadt, Wolfgang] Schott AG, Mainz, Germany. RP Contreras, MA (reprint author), Natl Renewable Energy Lab, Golden, CO USA. EM Miguel.contreras@nrel.gov RI Li, Jian/B-1627-2016 FU US Department of Energy [DE-AC36-08GO28308]; NREL FX The authors would like to thank Clay DeHart, Marty Scott, and Carolyn Beal for their work in processing the solar cells made for this work. This work was supported by the US Department of Energy under Contract No. DE-AC36-08GO28308 with NREL. NR 16 TC 66 Z9 66 U1 4 U2 107 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1062-7995 J9 PROG PHOTOVOLTAICS JI Prog. Photovoltaics PD NOV PY 2012 VL 20 IS 7 BP 843 EP 850 DI 10.1002/pip.2244 PG 8 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA 023YZ UT WOS:000310075200002 ER PT J AU Lee, HY Doudna, JA AF Lee, Ho Young Doudna, Jennifer A. TI TRBP alters human precursor microRNA processing in vitro SO RNA LA English DT Article DE RNAi; Dicer; TRBP; miRNA; post-transcriptional gene silencing ID RNA-BINDING PROTEIN; PASSENGER-STRAND; TUMOR-SUPPRESSOR; EXPRESSION; COMPLEX; CANCER; DICER; TRANSLATION; CLEAVAGE; DOMAIN AB MicroRNAs play central roles in controlling gene expression in human cells. Sequencing data show that many miRNAs are produced at different levels and as multiple isoforms that can vary in length at their 5' or 3' ends, but the biogenesis and functional significance of these RNAs are largely unknown. We show here that the human trans-activation response (TAR) RNA binding protein (TRBP), a known molecular partner of the miRNA processing enzyme Dicer, changes the rates of pre-miRNA cleavage in an RNA-structure-specific manner. Furthermore, TRBP can trigger the generation of iso-miRNAs (isomiRs) that are longer than the canonical sequence by one nucleotide. We show that this change in miRNA processing site can alter guide strand selection, resulting in preferential silencing of a different mRNA target. These results implicate TRBP as a key regulator of miRNA processing and targeting in humans. C1 [Lee, Ho Young; Doudna, Jennifer A.] Univ Calif Berkeley, Dept Mol & Cell Biol, Berkeley, CA 94720 USA. [Doudna, Jennifer A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Doudna, Jennifer A.] Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA. [Doudna, Jennifer A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Doudna, JA (reprint author), Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA. EM doudna@berkeley.edu FU National Institutes of Health FX J.A.D. is a Howard Hughes Medical Institute Investigator. This work was funded in part by the National Institutes of Health. We thank all the Doudna laboratory members especially Cameron L. Noland for helpful discussions. We thank O.K. Yoon for help in sequence analysis. NR 36 TC 47 Z9 47 U1 1 U2 14 PU COLD SPRING HARBOR LAB PRESS, PUBLICATIONS DEPT PI COLD SPRING HARBOR PA 1 BUNGTOWN RD, COLD SPRING HARBOR, NY 11724 USA SN 1355-8382 EI 1469-9001 J9 RNA JI RNA PD NOV PY 2012 VL 18 IS 11 BP 2012 EP 2019 DI 10.1261/rna.035501.112 PG 8 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA 023TH UT WOS:000310058000006 PM 23006623 ER PT J AU Kim, J Civale, L Nazaretski, E Haberkorn, N Ronning, F Sefat, AS Tajima, T Moeckly, BH Thompson, JD Movshovich, R AF Kim, Jeehoon Civale, L. Nazaretski, E. Haberkorn, N. Ronning, F. Sefat, A. S. Tajima, T. Moeckly, B. H. Thompson, J. D. Movshovich, R. TI Direct measurement of the magnetic penetration depth by magnetic force microscopy SO SUPERCONDUCTOR SCIENCE & TECHNOLOGY LA English DT Article ID TEMPERATURE-DEPENDENCE; II SUPERCONDUCTORS; GAP FUNCTION; B-11 NMR; VORTICES; MGB2; ANISOTROPY; FILMS; YBA2CU3O6.95; NODES AB We present an experimental approach using magnetic force microscopy for measurements of the absolute value of the magnetic penetration depth lambda in superconductors. lambda is obtained in a simple and robust way without introducing any tip modeling procedure via direct comparison of the Meissner response curves for a material of interest to those measured for a reference sample. Using a well-characterized Nb film as a reference, we determine the absolute value of lambda in a Ba(Fe0.92Co0.08)(2)As-2 single crystal and a MgB2 thin film through a comparative experiment. Our apparatus features simultaneous loading of multiple samples, and allows straightforward measurement of the absolute value of lambda in superconducting thin film or single-crystal samples. C1 [Kim, Jeehoon; Civale, L.; Haberkorn, N.; Ronning, F.; Tajima, T.; Thompson, J. D.; Movshovich, R.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Nazaretski, E.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Sefat, A. S.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Moeckly, B. H.] Superconductor Technol Inc, Santa Barbara, CA 93111 USA. RP Kim, J (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM jeehoon@lanl.gov RI Kim, Jeehoon/K-3763-2012; Sefat, Athena/R-5457-2016; OI Kim, Jeehoon/0000-0002-5742-5347; Sefat, Athena/0000-0002-5596-3504; Ronning, Filip/0000-0002-2679-7957; Civale, Leonardo/0000-0003-0806-3113 FU US Department of Energy, Basic Energy Sciences, Division of Materials Sciences and Engineering (MFM); T Tajima DOE Early Career Award; US Department of Energy [DE-AC02-98CH10886]; Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division FX The authors thank Y Q Wang for the RBS measurement. Work at LANL was supported by the US Department of Energy, Basic Energy Sciences, Division of Materials Sciences and Engineering (MFM, data analysis and manuscript preparation), and by T Tajima 2010 DOE Early Career Award (SQUID measurements). Work at Brookhaven (data analysis and manuscript preparation) was supported by the US Department of Energy under Contract No. DE-AC02-98CH10886. BaFe2As2 samples were grown at Oak Ridge National Laboratory with the support of the Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. NH is member of CONICET (Argentina). NR 42 TC 12 Z9 12 U1 3 U2 39 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-2048 J9 SUPERCOND SCI TECH JI Supercond. Sci. Technol. PD NOV PY 2012 VL 25 IS 11 AR 112001 DI 10.1088/0953-2048/25/11/112001 PG 6 WC Physics, Applied; Physics, Condensed Matter SC Physics GA 022KY UT WOS:000309959500001 ER PT J AU Roy, SB Chandra, LSS Chattopadhyay, MK Tiwari, MK Lodha, GS Myneni, GR AF Roy, S. B. Chandra, L. S. Sharath Chattopadhyay, M. K. Tiwari, M. K. Lodha, G. S. Myneni, G. R. TI A study on the effect of tantalum-impurity content on the superconducting properties of niobium materials used for making superconducting radio frequency cavities SO SUPERCONDUCTOR SCIENCE & TECHNOLOGY LA English DT Article ID HIGH-PURITY NIOBIUM; STRIPS; OXYGEN; TESLA AB Niobium materials in highly pure form are used in the fabrication of superconducting radio frequency cavities. We present here a study of the superconducting properties of such niobium materials that have been used in the fabrication of high accelerating gradient superconducting radio frequency cavities after determining their tantalum-impurity contents using a synchrotron-based x-ray fluorescence spectroscopy technique. Our results show that there is a small change in superconducting parameters such as T-C; H-C1 and H-C2 when the tantalum-impurity content varies from approximate to 150 to approximate to 1300 ppm. In contrast, a buffered chemical polishing of the same niobium samples changes all these superconducting parameters more significantly. The implications of these results on the performance of niobium superconducting radio frequency cavities are discussed. C1 [Roy, S. B.; Chandra, L. S. Sharath; Chattopadhyay, M. K.] Raja Ramanna Ctr Adv Technol, Magnet & Superconducting Mat Sect, Mat & Adv Accelerator Sci Div, Indore 452013, India. [Tiwari, M. K.; Lodha, G. S.] Raja Ramanna Ctr Adv Technol, Ind Synchrotron Utilizat Div, Xray Opt Sect, Indore 452013, India. [Myneni, G. R.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. RP Roy, SB (reprint author), Raja Ramanna Ctr Adv Technol, Magnet & Superconducting Mat Sect, Mat & Adv Accelerator Sci Div, Indore 452013, India. EM sbroy@rrcat.gov.in OI , Sharath Chandra/0000-0002-1253-6035 FU US DOE [DE-AC05-84ER40150]; Reference Metals Company Inc. [CRADA 2004-S002-Mod 2] FX The authors would like to thank Dr P D Gupta, Director, Raja Ramanna Centre for Advanced Technology for his keen interest and encouragement in the present work. One of the authors (GRM) is supported in part by US DOE contract DE-AC05-84ER40150 and Reference Metals Company Inc. CRADA 2004-S002-Mod 2. NR 42 TC 2 Z9 2 U1 0 U2 6 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-2048 EI 1361-6668 J9 SUPERCOND SCI TECH JI Supercond. Sci. Technol. PD NOV PY 2012 VL 25 IS 11 AR 115020 DI 10.1088/0953-2048/25/11/115020 PG 11 WC Physics, Applied; Physics, Condensed Matter SC Physics GA 022KY UT WOS:000309959500023 ER PT J AU Sinclair, JW Zuev, YL Cantoni, C Wee, SH Varanasi, C Thompson, JR Christen, DK AF Sinclair, J. W. Zuev, Y. L. Cantoni, C. Wee, S. H. Varanasi, C. Thompson, J. R. Christen, D. K. TI Matching field effects at tesla-level magnetic fields in critical current density in high-T-c superconductors containing self-assembled columnar defects SO SUPERCONDUCTOR SCIENCE & TECHNOLOGY LA English DT Article ID HIGH-TEMPERATURE SUPERCONDUCTORS; YBA2CU3O7 THIN-FILMS; II SUPERCONDUCTORS; TRANSPORT CURRENTS; BOSON LOCALIZATION; COATED CONDUCTORS; FLUX VORTICES; VORTEX; CRYSTALS; ARRAYS AB We have investigated the superconductive transport properties of YBa2Cu3O7 films containing self-assembled columnar arrays of second phase SrZrO3 or BaSnO3 precipitates. A matching condition between columnar pinning sites (aligned at or near the c axis) and external magnetic flux, tilted with respect to them, is identified in the critical current J(C)(H) data. The results for the material containing SrZrO3-based pins are analyzed within a simple intuitive model. At matching, the critical current is enhanced above the model prediction. In complementary contact-free investigations of BaSnO3-doped material, matching effects are observed over a wide range of temperatures in the field dependence of J(C)(H). The deduced matching fields agree reasonably well with the densities of columnar pins directly observed by scanning electron microscopy. C1 [Sinclair, J. W.; Zuev, Y. L.; Thompson, J. R.] Univ Tennessee, Dept Phys, Knoxville, TN 37996 USA. [Cantoni, C.; Wee, S. H.; Thompson, J. R.; Christen, D. K.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Varanasi, C.] Univ Dayton, Res Inst, Dayton, OH 45469 USA. RP Sinclair, JW (reprint author), Univ Tennessee, Dept Phys, Knoxville, TN 37996 USA. EM ylzuev@gmail.com RI Sinclair, John/E-7692-2011; Cantoni, Claudia/G-3031-2013 OI Cantoni, Claudia/0000-0002-9731-2021 FU Department of Energy, Office of Basic Energy Sciences-Division of Materials Sciences and Engineering; Office of Electricity Delivery and Energy Reliability (OE); AFOSR FX Work of JWS was sponsored by the Department of Energy, Office of Basic Energy Sciences-Division of Materials Sciences and Engineering; Work of YLZ, SHW, CC, JRT, and DKC was supported by the Office of Electricity Delivery and Energy Reliability (OE). Work of CV was sponsored by the AFOSR. This research was performed at the Oak Ridge National Laboratory, managed by UT-Battelle, LLC for the USDOE. NR 46 TC 0 Z9 0 U1 2 U2 18 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-2048 J9 SUPERCOND SCI TECH JI Supercond. Sci. Technol. PD NOV PY 2012 VL 25 IS 11 AR 115003 DI 10.1088/0953-2048/25/11/115003 PG 10 WC Physics, Applied; Physics, Condensed Matter SC Physics GA 022KY UT WOS:000309959500006 ER PT J AU Chang, JC Kovtun, O Blakely, RD Rosenthal, SJ AF Chang, Jerry C. Kovtun, Oleg Blakely, Randy D. Rosenthal, Sandra J. TI Labeling of neuronal receptors and transporters with quantum dots SO WILEY INTERDISCIPLINARY REVIEWS-NANOMEDICINE AND NANOBIOTECHNOLOGY LA English DT Review ID LIVING CELLS; LIVE CELLS; IN-VIVO; SEMICONDUCTOR NANOCRYSTALS; LATERAL MOBILITY; BIOTIN-BINDING; SURFACE TRAFFICKING; DIFFUSION DYNAMICS; GLYCINE RECEPTORS; TYPE-1 RECEPTOR AB The ability to efficiently visualize protein targets in cells is a fundamental goal in biological research. Recently, quantum dots (QDots) have emerged as a powerful class of fluorescent probes for labeling membrane proteins in living cells because of breakthrough advances in QDot surface chemistry and biofunctionalization strategies. This review discusses the increasing use of QDots for fluorescence imaging of neuronal receptors and transporters. The readers are briefly introduced to QDot structure, photophysical properties, and common synthetic routes toward the generation of water-soluble QDots. The following section highlights several reports of QDot application that seek to unravel molecular aspects of neuronal receptor and transporter regulation and trafficking. This article is closed with a prospectus of the future of derivatized QDots in neurobiological and pharmacological research. WIREs Nanomed Nanobiotechnol 2012, 4:605619. doi: 10.1002/wnan.1186 For further resources related to this article, please visit the WIREs website. C1 [Chang, Jerry C.; Kovtun, Oleg; Rosenthal, Sandra J.] Vanderbilt Univ, Dept Chem, Nashville, TN 37212 USA. [Blakely, Randy D.; Rosenthal, Sandra J.] Vanderbilt Univ, Dept Pharmacol, Nashville, TN USA. [Blakely, Randy D.] Vanderbilt Univ, Dept Psychiat, Nashville, TN USA. [Blakely, Randy D.] Vanderbilt Univ, Vanderbilt Brain Inst, Nashville, TN USA. [Blakely, Randy D.] Vanderbilt Univ, Silvio O Conte Ctr Neurosci Res, Nashville, TN USA. [Rosenthal, Sandra J.] Vanderbilt Univ, Dept Chem & Biomol Engn, Nashville, TN USA. [Rosenthal, Sandra J.] Vanderbilt Univ, Dept Phys & Astron, Nashville, TN 37235 USA. [Rosenthal, Sandra J.] Vanderbilt Univ, Vanderbilt Inst Nanoscale Sci & Engn, Nashville, TN USA. [Rosenthal, Sandra J.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN USA. RP Rosenthal, SJ (reprint author), Vanderbilt Univ, Dept Chem, Nashville, TN 37212 USA. EM sandra.j.rosenthal@vanderbilt.edu FU Vanderbilt Institute of Nanoscale Science and Engineering (VINSE); US National Institute of Health [EB003728, GM72048, MH07802, MH094527] FX J.C.C. acknowledges a research fellowship from the Vanderbilt Institute of Nanoscale Science and Engineering (VINSE). This work was supported by the US National Institute of Health (EB003728, GM72048, MH07802, and MH094527). NR 82 TC 9 Z9 10 U1 2 U2 35 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1939-5116 J9 WIRES NANOMED NANOBI JI Wiley Interdiscip. Rev.-Nanomed. Nanobiotechnol. PD NOV-DEC PY 2012 VL 4 IS 6 BP 605 EP 619 DI 10.1002/wnan.1186 PG 15 WC Nanoscience & Nanotechnology; Medicine, Research & Experimental SC Science & Technology - Other Topics; Research & Experimental Medicine GA 021VD UT WOS:000309912600002 PM 22887823 ER PT J AU Cruz-Martinez, K Rosling, A Zhang, Y Song, MZ Andersen, GL Banfield, JF AF Cruz-Martinez, Karelyn Rosling, Anna Zhang, Yang Song, Mingzhou Andersen, Gary L. Banfield, Jillian F. TI Effect of Rainfall-Induced Soil Geochemistry Dynamics on Grassland Soil Microbial Communities SO APPLIED AND ENVIRONMENTAL MICROBIOLOGY LA English DT Article ID CALIFORNIA ANNUAL GRASSLAND; NITROGEN LIMITATION; DIVERSITY; CARBON; RESPONSES; BIOMASS; MICROORGANISMS; WATER; VARIABILITY; COMPETITION AB In Mediterranean-type grassland ecosystems, the timing of rainfall events controls biogeochemical cycles, as well as the phenology and productivity of plants and animals. Here, we investigate the effect of short-term (days) soil environmental conditions on microbial community structure and composition during a natural wetting and drying cycle. Soil samples were collected from a meadow in Northern California at four time points after the first two rainfall events of the rainy season. We used 16S rRNA microarrays (PhyloChip) to track changes in bacterial and archaeal community composition. Microbial communities at time points 1 and 3 were significantly different than communities at time points 2 and 4. Based on ordination analysis, the available carbon, soil moisture, and temperature explained most of the variation in community structure. For the first time, a complementary and more comprehensive approach using linear regression and generalized logical networks were used to identify linear and nonlinear associations among environmental variables and with the relative abundance of subfamilies. Changes in soil moisture and available carbon were correlated with the relative abundance of many phyla. Only the phylum Actinobacteria showed a lineage-specific relationship to soil moisture but not to carbon or nitrogen. The results indicate that the use of a high taxonomic rank in correlations with nutritional indicators might obscure divergent subfamily-level responses to environmental parameters. An important implication of this research is that there is short-term variation in microbial community composition driven in part by rainfall fluctuation that may not be evident in long-term studies with coarser time resolution. C1 [Cruz-Martinez, Karelyn] Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. [Cruz-Martinez, Karelyn; Rosling, Anna] Swedish Univ Agr Sci, Dept Forest Mycol & Pathol, Uppsala BioCtr, S-75007 Uppsala, Sweden. [Zhang, Yang; Song, Mingzhou] New Mexico State Univ, Dept Comp Sci, Las Cruces, NM 88003 USA. [Andersen, Gary L.; Banfield, Jillian F.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Dept Ecol, Berkeley, CA 94720 USA. [Banfield, Jillian F.] Univ Calif Berkeley, Environm Sci Policy Dept, Berkeley, CA 94720 USA. [Banfield, Jillian F.] Univ Calif Berkeley, Dept Management, Berkeley, CA 94720 USA. [Banfield, Jillian F.] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. [Rosling, Anna] Indiana Univ, Dept Biol, Bloomington, IN USA. RP Cruz-Martinez, K (reprint author), Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. EM karelyn37@gmail.com RI Andersen, Gary/G-2792-2015; Rosling, Anna/D-1984-2012; OI Andersen, Gary/0000-0002-1618-9827; Song, Mingzhou/0000-0002-6883-6547 FU U.S. Department of Energy by the University of California, Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; National Centre for Earth and Surface Dynamics (USA); California Agricultural and Experiment Station; FORMAS; KVA; KSLA; Magn Bergwalls Foundation, Sweden FX Part of this work was performed under the auspices of the U.S. Department of Energy by the University of California, Lawrence Berkeley National Laboratory, under contract DE-AC02-05CH11231. Funding was provided by the National Centre for Earth and Surface Dynamics (USA) and the California Agricultural and Experiment Station. Additional support was provided by the FORMAS, KVA, KSLA, and Magn Bergwalls Foundation, Sweden. NR 59 TC 8 Z9 9 U1 2 U2 51 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 0099-2240 J9 APPL ENVIRON MICROB JI Appl. Environ. Microbiol. PD NOV PY 2012 VL 78 IS 21 BP 7587 EP 7595 DI 10.1128/AEM.00203-12 PG 9 WC Biotechnology & Applied Microbiology; Microbiology SC Biotechnology & Applied Microbiology; Microbiology GA 018RB UT WOS:000309678600011 PM 22904056 ER PT J AU Yi, S Seth, EC Men, YJ Stabler, SP Allen, RH Alvarez-Cohen, L Taga, ME AF Yi, Shan Seth, Erica C. Men, Yu-Jie Stabler, Sally P. Allen, Robert H. Alvarez-Cohen, Lisa Taga, Michiko E. TI Versatility in Corrinoid Salvaging and Remodeling Pathways Supports Corrinoid-Dependent Metabolism in Dehalococcoides mccartyi SO APPLIED AND ENVIRONMENTAL MICROBIOLOGY LA English DT Article ID ETHENOGENES STRAIN 195; TRANSCRIPTOMIC MICROARRAY ANALYSIS; MOLECULAR CHARACTERIZATION; REDUCTIVE DECHLORINATION; SALMONELLA-TYPHIMURIUM; COBALAMIN ANALOGS; GENOME SEQUENCE; VINYL-CHLORIDE; GROWTH; VITAMIN-B-12 AB Corrinoids are cobalt-containing molecules that function as enzyme cofactors in a wide variety of organisms but are produced solely by a subset of prokaryotes. Specific corrinoids are identified by the structure of their axial ligands. The lower axial ligand of a corrinoid can be a benzimidazole, purine, or phenolic compound. Though it is known that many organisms obtain corrinoids from the environment, the variety of corrinoids that can serve as cofactors for any one organism is largely unstudied. Here, we examine the range of corrinoids that function as cofactors for corrinoid-dependent metabolism in Dehalococcoides mccartyi strain 195. Dehalococcoides bacteria play an important role in the bioremediation of chlorinated solvents in the environment because of their unique ability to convert the common groundwater contaminants perchloroethene and trichloroethene to the innocuous end product ethene. All isolated D. mccartyi strains require exogenous corrinoids such as vitamin B-12 for growth. However, like many other corrinoid-dependent bacteria, none of the well-characterized D. mccartyi strains has been shown to be capable of synthesizing corrinoids de novo. In this study, we investigate the ability of D. mccartyi strain 195 to use specific corrinoids, as well as its ability to modify imported corrinoids to a functional form. We show that strain 195 can use only specific corrinoids containing benzimidazole lower ligands but is capable of remodeling other corrinoids by lower ligand replacement when provided a functional benzimidazole base. This study of corrinoid utilization and modification by D. mccartyi provides insight into the array of strategies that microorganisms employ in acquiring essential nutrients from the environment. C1 [Seth, Erica C.; Taga, Michiko E.] Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. [Yi, Shan; Men, Yu-Jie; Alvarez-Cohen, Lisa] Univ Calif Berkeley, Dept Civil & Environm Engn, Berkeley, CA 94720 USA. [Stabler, Sally P.; Allen, Robert H.] Univ Colorado, Dept Med, Div Hematol, Aurora, CO USA. [Alvarez-Cohen, Lisa] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Taga, ME (reprint author), Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. EM taga@berkeley.edu RI Yi, Shan/I-4589-2012 OI Yi, Shan/0000-0003-1371-0418 FU NIH grant [R00-GM083303]; NSF grant [MCB1122046]; NIEHS Superfund Basic Research Program [ES04705-19]; Strategic Environmental Research and Development Program [ER-1587]; NSF predoctoral fellowship FX This work was supported by NIH grant R00-GM083303 and NSF grant MCB1122046 to M.E.T., the NIEHS Superfund Basic Research Program ES04705-19 and the Strategic Environmental Research and Development Program ER-1587 to L.A.-C., and an NSF predoctoral fellowship to E.C.S. NR 56 TC 30 Z9 30 U1 1 U2 26 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 0099-2240 J9 APPL ENVIRON MICROB JI Appl. Environ. Microbiol. PD NOV PY 2012 VL 78 IS 21 BP 7745 EP 7752 DI 10.1128/AEM.02150-12 PG 8 WC Biotechnology & Applied Microbiology; Microbiology SC Biotechnology & Applied Microbiology; Microbiology GA 018RB UT WOS:000309678600028 PM 22923412 ER PT J AU Yeh, HH Chiang, YM Entwistle, R Ahuja, M Lee, KH Bruno, KS Wu, TK Oakley, BR Wang, CCC AF Yeh, Hsu-Hua Chiang, Yi-Ming Entwistle, Ruth Ahuja, Manmeet Lee, Kuan-Han Bruno, Kenneth S. Wu, Tung-Kung Oakley, Berl R. Wang, Clay C. C. TI Molecular genetic analysis reveals that a nonribosomal peptide synthetase-like (NRPS-like) gene in Aspergillus nidulans is responsible for microperfuranone biosynthesis SO APPLIED MICROBIOLOGY AND BIOTECHNOLOGY LA English DT Article DE Aspergillus nidulans; Nonribosomal peptide synthetase-like; Microperfuranone; Biosynthesis ID CLUSTER; POLYKETIDE; DISCOVERY; PATHWAY; ORYZAE; CONSTITUENTS; ALKALOIDS; FUMIGATUS; PRECURSOR; PROTEINS AB Genome sequencing of Aspergillus species including Aspergillus nidulans has revealed that there are far more secondary metabolite biosynthetic gene clusters than secondary metabolites isolated from these organisms. This implies that these organisms can produce additional secondary metabolites, which have not yet been elucidated. The A. nidulans genome contains 12 nonribosomal peptide synthetase (NRPS), one hybrid polyketide synthase/NRPS, and 14 NRPS-like genes. The only NRPS-like gene in A. nidulans with a known product is tdiA, which is involved in terrequinone A biosynthesis. To attempt to identify the products of these NRPS-like genes, we replaced the native promoters of the NRPS-like genes with the inducible alcohol dehydrogenase (alcA) promoter. Our results demonstrated that induction of the single NRPS-like gene AN3396.4 led to the enhanced production of microperfuranone. Furthermore, heterologous expression of AN3396.4 in Aspergillus niger confirmed that only one NRPS-like gene, AN3396.4, is necessary for the production of microperfuranone. C1 [Yeh, Hsu-Hua; Wu, Tung-Kung] Natl Chiao Tung Univ, Dept Biol Sci & Technol, Hsinchu 30010, Taiwan. [Yeh, Hsu-Hua; Chiang, Yi-Ming; Wang, Clay C. C.] Univ So Calif, Sch Pharm, Dept Pharmacol & Pharmaceut Sci, Los Angeles, CA 90089 USA. [Chiang, Yi-Ming; Lee, Kuan-Han] Chia Nan Univ Pharm & Sci, Grad Inst Pharmaceut Sci, Tainan 71710, Taiwan. [Entwistle, Ruth; Ahuja, Manmeet; Oakley, Berl R.] Univ Kansas, Dept Mol Biosci, Lawrence, KS 66045 USA. [Bruno, Kenneth S.] Pacific NW Natl Lab, Chem & Biol Proc Dev Grp, Energy & Environm Directorate, Richland, WA 99352 USA. [Wang, Clay C. C.] Univ So Calif, Dept Chem, Dornsife Coll Letters Arts & Sci, Los Angeles, CA 90089 USA. RP Wang, CCC (reprint author), Univ So Calif, Sch Pharm, Dept Pharmacol & Pharmaceut Sci, 1985 Zonal Ave, Los Angeles, CA 90089 USA. EM clayw@usc.edu OI Chiang, Yi-Ming/0000-0001-9899-1364; Oakley, Berl/0000-0002-3046-8240 FU National Institute of General Medical Sciences [PO1GM084077]; PNNL Energy and Environment Directorate's Laboratory Directed Research and Development office FX This project was supported by grant PO1GM084077 from the National Institute of General Medical Sciences. Research conducted at the Pacific Northwest National Lab was supported by the PNNL Energy and Environment Directorate's Laboratory Directed Research and Development office. The content is solely the responsibility of the authors and does not necessarily represent the official views of the National Institute of General Medical Sciences or the National Institutes of Health. NR 34 TC 21 Z9 34 U1 2 U2 44 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0175-7598 J9 APPL MICROBIOL BIOT JI Appl. Microbiol. Biotechnol. PD NOV PY 2012 VL 96 IS 3 BP 739 EP 748 DI 10.1007/s00253-012-4098-9 PG 10 WC Biotechnology & Applied Microbiology SC Biotechnology & Applied Microbiology GA 019AI UT WOS:000309708900013 PM 22627757 ER PT J AU Weidner, JW Mashnik, SG John, KD Ballard, B Birnbaum, ER Bitteker, LJ Couture, A Fassbender, ME Goff, GS Gritzo, R Hemez, FM Runde, W Ullmann, JL Wolfsberg, LE Nortier, FM AF Weidner, J. W. Mashnik, S. G. John, K. D. Ballard, B. Birnbaum, E. R. Bitteker, L. J. Couture, A. Fassbender, M. E. Goff, G. S. Gritzo, R. Hemez, F. M. Runde, W. Ullmann, J. L. Wolfsberg, L. E. Nortier, F. M. TI Ac-225 and Ra-223 production via 800 MeV proton irradiation of natural thorium targets SO APPLIED RADIATION AND ISOTOPES LA English DT Article DE Actinium-225; Radium-223; Cross section; Yield; Proton irradiation; Thorium target ID TOTAL CROSS-SECTIONS; ENERGY-RANGE; NA-22; THERAPY; BE-7; RADIOIMMUNOTHERAPY; ACTINIUM-225; AL-27 AB Cross sections for the formation of Ac-225,Ac-227, Ra-223,Ra-225, and Th-227 via the proton bombardment of natural thorium targets were measured at a nominal proton energy of 800 MeV. No earlier experimental cross section data for the production of Ra-223,Ra-225, Ac-227 and Th-227 by this method were found in the literature. A comparison of theoretical predictions with the experimental data shows agreement within a factor of two. Results indicate that accelerator-based production of Ac-225 and Ra-223 is a viable production method. Published by Elsevier Ltd. C1 [Weidner, J. W.; Mashnik, S. G.; John, K. D.; Ballard, B.; Birnbaum, E. R.; Bitteker, L. J.; Couture, A.; Fassbender, M. E.; Goff, G. S.; Gritzo, R.; Hemez, F. M.; Runde, W.; Ullmann, J. L.; Wolfsberg, L. E.; Nortier, F. M.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Weidner, JW (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM john.weidner@us.army.mil; meiring@lanl.gov RI Ballard, Beau/E-2925-2017; OI Ballard, Beau/0000-0003-1206-9358; John, Kevin/0000-0002-6181-9330 FU United States Department of Energy Office of Science from Isotope Development and Production for Research and Applications subprogram in the Office of Nuclear Physics FX We gratefully acknowledge funding by the United States Department of Energy Office of Science via an award from The Isotope Development and Production for Research and Applications subprogram in the Office of Nuclear Physics. We are also very thankful for the technical assistance provided by members of the LANL C-NR and C-IIAC groups, members of the AOT-OPS group, and the LANSCE-WNR staff. NR 36 TC 15 Z9 15 U1 1 U2 23 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0969-8043 J9 APPL RADIAT ISOTOPES JI Appl. Radiat. Isot. PD NOV PY 2012 VL 70 IS 11 BP 2590 EP 2595 DI 10.1016/j.apradiso.2012.07.003 PG 6 WC Chemistry, Inorganic & Nuclear; Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical Imaging SC Chemistry; Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical Imaging GA 020CU UT WOS:000309787100006 PM 22944532 ER PT J AU Weidner, JW Mashnik, SG John, KD Hemez, F Ballard, B Bach, H Birnbaum, ER Bitteker, LJ Couture, A Dry, D Fassbender, ME Gulley, MS Jackman, KR Ullmann, JL Wolfsberg, LE Nortier, FM AF Weidner, J. W. Mashnik, S. G. John, K. D. Hemez, F. Ballard, B. Bach, H. Birnbaum, E. R. Bitteker, L. J. Couture, A. Dry, D. Fassbender, M. E. Gulley, M. S. Jackman, K. R. Ullmann, J. L. Wolfsberg, L. E. Nortier, F. M. TI Proton-induced cross sections relevant to production of Ac-225 and Ra-223 in natural thorium targets below 200 MeV SO APPLIED RADIATION AND ISOTOPES LA English DT Article DE Actinium-225; Radium-223; Cross section; Yield; Proton irradiation; Thorium target ID SPALLATION; NUCLIDES; THERAPY AB Cross sections for Ra-223,Ra-225, Ac-225 and Th-227 production by the proton bombardment of natural thorium targets were measured at proton energies below 200 MeV. Our measurements are in good agreement with previously published data and offer a complete excitation function for Ra-223,Ra-225 in the energy range above 90 MeV. Comparison of theoretical predictions with the experimental data shows reasonable-to-good agreement. Results indicate that accelerator-based production of Ac-225 and Ra-223 below 200 MeV is a viable production method. Published by Elsevier Ltd. C1 [Weidner, J. W.; Mashnik, S. G.; John, K. D.; Hemez, F.; Ballard, B.; Bach, H.; Birnbaum, E. R.; Bitteker, L. J.; Couture, A.; Dry, D.; Fassbender, M. E.; Gulley, M. S.; Jackman, K. R.; Ullmann, J. L.; Wolfsberg, L. E.; Nortier, F. M.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Weidner, JW (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM john.weidner@us.army.mil; meiring@lanl.gov RI Ballard, Beau/E-2925-2017; OI Ballard, Beau/0000-0003-1206-9358; John, Kevin/0000-0002-6181-9330 FU United States Department of Energy Office of Science from Isotope Development and Production for Research and Applications subprogram in the Office of Nuclear Physics FX The authors gratefully acknowledge funding by the United States Department of Energy Office of Science via an award from The Isotope Development and Production for Research and Applications subprogram in the Office of Nuclear Physics. They are also very thankful for the technical assistance provided by members of the LANL C-NR and C-IIAC groups, members of the LANSCE AOT-OPS group, and the LANSCE-WNR staff. NR 29 TC 15 Z9 15 U1 0 U2 18 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0969-8043 J9 APPL RADIAT ISOTOPES JI Appl. Radiat. Isot. PD NOV PY 2012 VL 70 IS 11 BP 2602 EP 2607 DI 10.1016/j.apradiso.2012.07.006 PG 6 WC Chemistry, Inorganic & Nuclear; Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical Imaging SC Chemistry; Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical Imaging GA 020CU UT WOS:000309787100008 PM 22940414 ER PT J AU McClellan, AC Luthi, JC Lynch, JR Soucie, JM Kulkarni, R Guasch, A Huff, ED Gilbertson, D McClellan, WM DeBaun, MR AF McClellan, Ann C. Luthi, Jean-Christophe Lynch, Janet R. Soucie, J. Michael Kulkarni, Roshni Guasch, Antonio Huff, Edwin D. Gilbertson, David McClellan, William M. DeBaun, Michael R. TI High one year mortality in adults with sickle cell disease and end-stage renal disease SO BRITISH JOURNAL OF HAEMATOLOGY LA English DT Article DE sickle cell disease; kidney disease; end-stage renal disease; mortality; disparities ID HEMODIALYSIS-PATIENTS; RISK-FACTORS; CHILDREN; DEATH; US AB Adequate pre-dialysis care reduces mortality among end-stage renal disease (ESRD) patients.We tested thehypothesis that individuals with ESRD due to sickle cell disease (SCDESRD) receiving pre-ESRD care have lower mortality compared to individuals without pre-ESRD care.We examined the association between mortality and pre-ESRD care in incident SCDESRD patients who started haemodialysis between 1 June, 2005 and 31 May, 2009using data provided by the Centers for Medicare and MedicaidServices (CMS).SCDESRD was reported for 410 (0.1%) of 442017 patients. One year after starting dialysis, 108 (26.3%) patients with incident ESRD attributed to SCD died; the hazard ratio (HR) for mortality among patients with SCDESRD compared to those without SCD as the primary cause of renal failure was 2.80 (95% confidence interval [CI] 2.313.38). Patients with SCDESRD receiving pre-dialysis nephrology care had a lower death rate than those with SCDESRD who did not receive pre-dialysis nephrology care (HR=0.67, 95% CI 0.450.99). The one-year mortality rate following an ESRD diagnosis was almost three times higher in individuals with SCD when compared to those without SCD but with ESRD and could be attenuated by pre-dialysis nephrology care. C1 [DeBaun, Michael R.] Vanderbilt Univ, Dept Pediat, Div Hematol Oncol, Nashville, TN 37232 USA. [Gilbertson, David] USRDS, Minneapolis, MN USA. [Huff, Edwin D.] Ctr Medicare Serv, Boston, MA USA. [Huff, Edwin D.] Ctr Medicaid Serv, Boston, MA USA. [Kulkarni, Roshni] Michigan State Univ, E Lansing, MI 48824 USA. [Lynch, Janet R.] Midatlantic Renal Coalit, Richmond, VA USA. [Luthi, Jean-Christophe] CHU Vaudois, Inst Social & Prevent Med IUMSP, Epalinges, Switzerland. [Luthi, Jean-Christophe] Univ Lausanne, CH-1066 Epalinges, Switzerland. [Luthi, Jean-Christophe; Guasch, Antonio; McClellan, William M.] Emory Univ, Atlanta, GA 30322 USA. [McClellan, Ann C.] Oak Ridge Inst Sci & Educ, Oak Ridge, TN USA. [McClellan, Ann C.; Soucie, J. Michael; Kulkarni, Roshni] Ctr Dis Control & Prevent, Atlanta, GA USA. RP DeBaun, MR (reprint author), Vanderbilt Univ, Dept Pediat, Div Hematol Oncol, 2200 Childrens Way,DOT 11206, Nashville, TN 37232 USA. EM m.debaun@vanderbilt.edu FU Centers for Medicare and Medicaid Services (CMS), Department of Health and Human Services" [HHSM-500-2010-005C] FX The analyses upon which this publication is based were performed under Contract Number HHSM-500-2010-005C, entitled 'End Stage Renal Disease Networks Organization Number 5", sponsored by the Centers for Medicare and Medicaid Services (CMS), Department of Health and Human Services." This article is a direct result of the Health Care Quality Improvement Program initiated by CMS, which has encouraged identification of quality improvement projects derived from analysis of patterns of care, and therefore required no special funding on the part of this contractor. This research was supported in part by an appointment to the Research Participation Program at the Centers for Disease Control and Prevention, Division of Blood Disorders administered by the Oak Ridge Institute for Science and Education through an interagency agreement between the U. S. Department of Energy and the Centers for Disease Control and Prevention. The findings and conclusions in this report are those of the authors and do not necessarily represent the official position of the Centers for Disease Control and Prevention. We thank Dr. Steven Embury and Mrs. Deborah Jones for reviewing and editing the manuscript. NR 13 TC 28 Z9 28 U1 0 U2 3 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0007-1048 J9 BRIT J HAEMATOL JI Br. J. Haematol. PD NOV PY 2012 VL 159 IS 3 BP 360 EP 367 DI 10.1111/bjh.12024 PG 8 WC Hematology SC Hematology GA 019DO UT WOS:000309717500012 PM 22967259 ER PT J AU Katz, MJ Riha, SC Jeong, NC Martinson, ABF Farha, OK Hupp, JT AF Katz, Michael J. Riha, Shannon C. Jeong, Nak Cheon Martinson, Alex B. F. Farha, Omar K. Hupp, Joseph T. TI Toward solar fuels: Water splitting with sunlight and "rust"? SO COORDINATION CHEMISTRY REVIEWS LA English DT Review DE Hematite; Solar fuels; Alternative energy ID DRIVEN OXYGEN EVOLUTION; NANOSTRUCTURED ALPHA-FE2O3; HYDROGEN-PRODUCTION; HEMATITE ALPHA-FE2O3; DOPED HEMATITE; VISIBLE-LIGHT; PHOTOANODES; ELECTRODES; OXIDATION; FILMS AB Iron(III)oxide in the form of hematite is, in many respects, an attractive material for the photocatalytic production of molecular oxygen from water. Especially over the past six years, several developments have advanced the performance of water oxidation cells based on this material. Nevertheless, the best versions of these photoelectrodes produce only about a fifth of the maximum photocurrent (and dioxygen) theoretically obtainable, while operating at photovoltages also well short of the theoretical maximum. Here we describe the factors limiting the performance of hematite as a photo-catalyst and outline approaches that have been, or might be, tried to overcome them. These factors include low hole mobility, bulk charge recombination, surface charge recombination, slow water oxidation kinetics, and poor light absorption. Whether hematite will soon become a practical photo-catalyst for water oxidation is uncertain. But, the schemes developed and the lessons learned will likely prove transferrable to other candidate photocatalyst materials. (C) 2012 Elsevier BM. All rights reserved. C1 [Katz, Michael J.; Riha, Shannon C.; Jeong, Nak Cheon; Martinson, Alex B. F.; Farha, Omar K.; Hupp, Joseph T.] Northwestern Univ, Argonne NW Solar Energy Res ANSER Ctr, Evanston, IL 60208 USA. [Katz, Michael J.; Jeong, Nak Cheon; Farha, Omar K.; Hupp, Joseph T.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Hupp, Joseph T.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Riha, Shannon C.; Martinson, Alex B. F.; Hupp, Joseph T.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Hupp, JT (reprint author), Northwestern Univ, Argonne NW Solar Energy Res ANSER Ctr, 2145 Sheridan Rd, Evanston, IL 60208 USA. EM j-hupp@northwestern.edu RI Hupp, Joseph/K-8844-2012; Farha, Omar/B-5512-2014; Jeong, Nak Cheon/L-4082-2016; OI Hupp, Joseph/0000-0003-3982-9812; Farha, Omar/0000-0002-9904-9845; Jeong, Nak Cheon/0000-0003-3320-5750; Katz, Michael/0000-0002-7744-3956; Martinson, Alex/0000-0003-3916-1672 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001059]; U.S. Department of Energy Office of Science Laboratory [DE-AC02-06CH11357] FX We gratefully acknowledge the ANSER Center, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number DE-SC0001059, for support of our own work on hematite and photocatalysis. The electron microscopy was accomplished at the Electron Microscopy Center for Materials Research at Argonne National Laboratory, a U.S. Department of Energy Office of Science Laboratory operated under Contract No. DE-AC02-06CH11357 by UChicago Argonne, LLC. NR 65 TC 125 Z9 125 U1 6 U2 316 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0010-8545 J9 COORDIN CHEM REV JI Coord. Chem. Rev. PD NOV PY 2012 VL 256 IS 21-22 SI SI BP 2521 EP 2529 DI 10.1016/j.ccr.2012.06.017 PG 9 WC Chemistry, Inorganic & Nuclear SC Chemistry GA 021OS UT WOS:000309895800011 ER PT J AU Yue, DJ Khatav, P You, FQ Darling, SB AF Yue, Dajun Khatav, Prasad You, Fengqi Darling, Seth B. TI Deciphering the uncertainties in life cycle energy and environmental analysis of organic photovoltaics SO ENERGY & ENVIRONMENTAL SCIENCE LA English DT Article ID POLYMER SOLAR-CELLS; SOLVENT-EXTRACTION; MODULES; INDIUM; ANODE; OXIDE; TEMPERATURE; ELECTRODES; EFFICIENT; PAYBACK AB Organic photovoltaic (OPV) technologies are rapidly emerging as a viable alternative for traditional silicon and thin film technologies. OPVs are projected to be comparatively inexpensive and have a low energy payback time (EPBT) with lower levels of anthropogenic emissions during their lifetime. In this paper, we have analyzed the life cycle environmental impacts and EPBT of a scalable OPV module in the three cities Chicago, New York and San Francisco, for the current, near-term future and long-term future scenarios. Instead of using the deterministic or 'single point estimate' method, we employed a probabilistic approach by applying an uncertainty analysis to each of these scenarios using the Monte Carlo simulation method, and thereby quantifying the uncertainty and risk associated with each scenario. By comparing the proposed OPV technology with four typical silicon-based and thin-film photovoltaics in the aspects of EPBT and greenhouse gas (GHG) emissions, we demonstrate the great potential of OPVs in environmental sustainability. The probabilistic approach displayed a wide distribution for the EPBT and CO2 emission factor values, rather than squeezing around a single value. This demonstrated the insufficiency of deterministic analysis, which would give a false impression of certainty in the outcomes. C1 [Yue, Dajun; Khatav, Prasad; You, Fengqi] Northwestern Univ, Dept Chem & Biol Engn, Evanston, IL 60208 USA. [Darling, Seth B.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. [Darling, Seth B.] Univ Chicago, Inst Mol Engn, Chicago, IL 60637 USA. RP Yue, DJ (reprint author), Northwestern Univ, Dept Chem & Biol Engn, 2145 Sheridan Rd, Evanston, IL 60208 USA. EM you@northwestern.edu; darling@anl.gov RI You, Fengqi/F-6894-2011; You, Fengqi/B-5040-2011 OI You, Fengqi/0000-0001-9609-4299 FU Initiative for Sustainability and Energy at Northwestern (ISEN); Center for Nanoscale Materials, a U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility [DE-AC02-06CH11357] FX The authors gratefully acknowledge the financial support from the Initiative for Sustainability and Energy at Northwestern (ISEN). This work was performed, in part, at the Center for Nanoscale Materials, a U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences User Facility under Contract no. DE-AC02-06CH11357. NR 58 TC 50 Z9 50 U1 3 U2 43 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1754-5692 J9 ENERG ENVIRON SCI JI Energy Environ. Sci. PD NOV PY 2012 VL 5 IS 11 BP 9163 EP 9172 DI 10.1039/c2ee22597b PG 10 WC Chemistry, Multidisciplinary; Energy & Fuels; Engineering, Chemical; Environmental Sciences SC Chemistry; Energy & Fuels; Engineering; Environmental Sciences & Ecology GA 023AV UT WOS:000310006200002 ER PT J AU Greeley, J Markovic, NM AF Greeley, Jeffrey Markovic, Nenad M. TI The road from animal electricity to green energy: combining experiment and theory in electrocatalysis SO ENERGY & ENVIRONMENTAL SCIENCE LA English DT Review ID SINGLE-CRYSTAL ELECTRODES; FUEL-CELL ELECTROCATALYSTS; OXYGEN-REDUCTION ACTIVITY; ELECTROLYTIC HYDROGEN EVOLUTION; SCANNING-TUNNELING-MICROSCOPY; BIMETALLIC ALLOY SURFACES; ROTATING-DISK ELECTRODE; X-RAY-DIFFRACTION; IN-SITU FTIR; CO ELECTROOXIDATION AB Advances in the field of electrocatalysis over the past several decades have been driven both by improvements in fundamental techniques for probing the solid-liquid electrochemical interface and by the technological imperative to develop enhanced low temperature electrocatalytic devices. In this review, we describe how a synergistic interaction between fundamental science and technological progress has resulted in both the emergence of greatly enhanced understanding of electrocatalytic systems and the development of practically improved electrocatalysts. Since it is not possible to summarize in detail all relevant developments in this broad field in such a brief space, we focus selectively on the early historical development of the field and on the use of trends-based analyses to describe the properties of electrocatalytic materials in terms of relatively simple catalytic properties, or descriptors. We begin by discussing aspects of the historical development of "reversible fuel cells" in acidic media, including topics relevant both to fuel cells, wherein hydrogen and oxygen are converted to water with concomitant production of electricity (electrons), and to electrolyzers, wherein electrons are used to initiate water splitting to yield hydrogen and oxygen. We then show how this development has stimulated the development of in situ and ex situ surface sensitive probes and spectroscopic methods capable of elucidating fundamental (atomic-/molecular-level) chemical and electronic properties of electrode-electrolyte interfaces. We further discuss how enhanced computational approaches, that can accurately calculate covalent bonding interactions in these systems, have contributed to the growth of a synergistic experimental/computational approach to electrochemical surface science that has resulted in a highly successful paradigm for the understanding of reactivity trends across a space of different metals, alloys, and metal oxides; this work, in turn, has spurred the development of alternative energy systems for efficient conversion and storage of chemical energy. We conclude with a discussion of some further needs for methodological developments and future research directions. C1 [Greeley, Jeffrey] Argonne Natl Lab, Ctr Nanoscale Mat, Lemont, IL 60559 USA. [Markovic, Nenad M.] Argonne Natl Lab, Div Mat Sci, Lemont, IL 60559 USA. RP Greeley, J (reprint author), Argonne Natl Lab, Ctr Nanoscale Mat, Lemont, IL 60559 USA. EM jgreeley@anl.gov; markovic@anl.gov FU Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC0206CH11357]; Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences [DE-AC0206CH11357] FX J.G. acknowledges an Early Career grant from the Department of Energy, Office of Science, Office of Basic Energy Sciences, under contract DE-AC0206CH11357. N.M. acknowledges support from the Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences, under contract DE-AC0206CH11357. NR 170 TC 59 Z9 59 U1 10 U2 223 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1754-5692 EI 1754-5706 J9 ENERG ENVIRON SCI JI Energy Environ. Sci. PD NOV PY 2012 VL 5 IS 11 BP 9246 EP 9256 DI 10.1039/c2ee21754f PG 11 WC Chemistry, Multidisciplinary; Energy & Fuels; Engineering, Chemical; Environmental Sciences SC Chemistry; Energy & Fuels; Engineering; Environmental Sciences & Ecology GA 023AV UT WOS:000310006200008 ER PT J AU Huang, ZG Autrey, T AF Huang, Zhenguo Autrey, Tom TI Boron-nitrogen-hydrogen (BNH) compounds: recent developments in hydrogen storage, applications in hydrogenation and catalysis, and new syntheses SO ENERGY & ENVIRONMENTAL SCIENCE LA English DT Review ID AMMONIA BORANE DEHYDROGENATION; HIGH-EXTENT DEHYDROGENATION; ALKALI-METAL AMIDOBORANES; THERMAL-DECOMPOSITION; CRYSTAL-STRUCTURE; HYDRIDE TRANSFER; AMINE-BORANES; SPENT FUEL; DIBORANE; DIAMMONIATE AB The strong efforts devoted to the exploration of BNH compounds for hydrogen storage have led to impressive advances in the field of boron chemistry. This review summarizes progress in this field from three aspects. It starts with the most recent developments in using BNH compounds for hydrogen storage, covering NH3BH3, B3H8- containing compounds, and CBN compounds. The following section then highlights interesting applications of BNH compounds in hydrogenation and catalysis. The last part is focused on breakthroughs in the syntheses and discovery of new BNH organic analogues. The role of N-H delta+center dot center dot center dot H delta--B dihydrogen interactions in molecule packing, thermal hydrogen evolution, and syntheses is also discussed within the review. C1 [Huang, Zhenguo] Univ Wollongong, Inst Superconducting & Elect Mat, N Wollongong, NSW 2522, Australia. [Autrey, Tom] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. RP Huang, ZG (reprint author), Univ Wollongong, Inst Superconducting & Elect Mat, Innovation Campus,Squires Way, N Wollongong, NSW 2522, Australia. EM zhenguo@uow.edu.au; tom.autrey@pnnl.gov RI Huang, Zhenguo/F-4483-2016 FU Australian Research Council [DE120101496]; U.S. Department of Energy's Basic Energy Sciences, Division of Chemical Sciences, Biosciences and Geosciences FX Z.H. is the recipient of a Discovery Early Career Research Award conferred by the Australian Research Council (Project no. DE120101496). T.A. acknowledges support from the U.S. Department of Energy's Basic Energy Sciences, Division of Chemical Sciences, Biosciences and Geosciences. Pacific Northwest National Laboratory is operated by Battelle. NR 148 TC 90 Z9 91 U1 5 U2 165 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1754-5692 J9 ENERG ENVIRON SCI JI Energy Environ. Sci. PD NOV PY 2012 VL 5 IS 11 BP 9257 EP 9268 DI 10.1039/c2ee23039a PG 12 WC Chemistry, Multidisciplinary; Energy & Fuels; Engineering, Chemical; Environmental Sciences SC Chemistry; Energy & Fuels; Engineering; Environmental Sciences & Ecology GA 023AV UT WOS:000310006200009 ER EF