FN Thomson Reuters Web of Science™ VR 1.0 PT J AU Mohammed, I Saha, P Williams, LLR Liesenborgs, J Sebesta, K AF Mohammed, Irshad Saha, Prasenjit Williams, Liliya L. R. Liesenborgs, Jori Sebesta, Kevin TI Quantifying substructures in Hubble Frontier Field clusters: comparison with Lambda CDM simulations SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE galaxies: clusters: individual: Abell 2744; galaxies: clusters: individual: Abell 370; galaxies: clusters: individual: Abell S1063; galaxies: clusters: individual: MACS J0416; 1+2403; galaxies: clusters: individual: MACS J0717; 5+3745; galaxies: clusters: individual: MACS J1149; 5+2223 ID STRONG-LENSING ANALYSIS; DARK-MATTER; ABELL 2744; X-RAY; GALAXY CLUSTERS; COSMOLOGICAL SIMULATIONS; MAGNIFICATION MAPS; MACS J0416.1-2403; INTERNAL DYNAMICS; DENSITY PROFILES AB The Hubble Frontier Fields (HFFs) are six clusters of galaxies, all showing indications of recent mergers, which have recently been observed for lensed images. As such they are the natural laboratories to study the merging history of galaxy clusters. In this work, we explore the 2D power spectrum of the mass distribution P-M(k) as a measure of substructure. We compare P-M(k) of these clusters (obtained using strong gravitational lensing) to that of I > cold dark matter simulated clusters of similar mass. To compute lensing P-M(k), we produced free-form lensing mass reconstructions of HFF clusters, without any light traces mass (LTM) assumption. The inferred power at small scales tends to be larger if (i) the cluster is at lower redshift, and/or (ii) there are deeper observations and hence more lensed images. In contrast, lens reconstructions assuming LTM show higher power at small scales even with fewer lensed images; it appears the small-scale power in the LTM reconstructions is dominated by light information, rather than the lensing data. The average lensing derived P-M(k) shows lower power at small scales as compared to that of simulated clusters at redshift zero, both dark matter only and hydrodynamical. The possible reasons are (i) the available strong lensing data are limited in their effective spatial resolution on the mass distribution; (ii) HFF clusters have yet to build the small-scale power they would have at z similar to 0 or (iii) simulations are somehow overestimating the small-scale power. C1 [Mohammed, Irshad] Fermilab Natl Accelerator Lab, Theoret Astrophys Grp, POB 500, Batavia, IL 60510 USA. [Mohammed, Irshad; Saha, Prasenjit] Univ Zurich, Inst Phys, Winterthurerstr 190, CH-8057 Zurich, Switzerland. [Mohammed, Irshad; Saha, Prasenjit] Univ Zurich, Inst Computat Sci, Winterthurerstr 190, CH-8057 Zurich, Switzerland. [Williams, Liliya L. R.; Sebesta, Kevin] Univ Minnesota, Sch Phys & Astron, 116 Church St SE, Minneapolis, MN 55455 USA. [Liesenborgs, Jori] Univ Hasselt, Expertisectr Digitale Media, Wetenschapspk 2, B-3590 Diepenbeek, Belgium. RP Mohammed, I (reprint author), Fermilab Natl Accelerator Lab, Theoret Astrophys Grp, POB 500, Batavia, IL 60510 USA.; Mohammed, I (reprint author), Univ Zurich, Inst Phys, Winterthurerstr 190, CH-8057 Zurich, Switzerland.; Mohammed, I (reprint author), Univ Zurich, Inst Computat Sci, Winterthurerstr 190, CH-8057 Zurich, Switzerland. EM mohammed@fnal.gov FU Fermi Research Alliance, LLC [De-AC02-07CH11359]; United States Department of Energy FX IM is supported by Fermi Research Alliance, LLC under Contract No. De-AC02-07CH11359 with the United States Department of Energy. NR 73 TC 1 Z9 1 U1 2 U2 2 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD JUN 21 PY 2016 VL 459 IS 2 BP 1698 EP 1709 DI 10.1093/mnras/stw727 PG 12 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DO0LU UT WOS:000377471200043 ER PT J AU Koda, J Blake, C Beutler, F Kazin, E Marin, F AF Koda, Jun Blake, Chris Beutler, Florian Kazin, Eyal Marin, Felipe TI Fast and accurate mock catalogue generation for low-mass galaxies SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE methods: numerical; cosmology: theory; large-scale structure of Universe ID BARYON ACOUSTIC-OSCILLATIONS; DARK ENERGY SURVEY; LARGE-SCALE STRUCTURE; WIGGLEZ OVERLAP REGION; LUMINOUS RED GALAXIES; DIGITAL SKY SURVEY; 1ST DATA RELEASE; SPECTROSCOPIC SURVEY; POWER-SPECTRUM; HALO CATALOGS AB We present an accurate and fast framework for generating mock catalogues including low-mass haloes, based on an implementation of the COmoving Lagrangian Acceleration (COLA) technique. Multiple realisations of mock catalogues are crucial for analyses of large-scale structure, but conventional N-body simulations are too computationally expensive for the production of thousands of realizations. We show that COLA simulations can produce accurate mock catalogues with a moderate computation resource for low- to intermediate-mass galaxies in 10(12) M-aS (TM) haloes, both in real and redshift space. COLA simulations have accurate peculiar velocities, without systematic errors in the velocity power spectra for k a parts per thousand currency sign 0.15 h Mpc(-1), and with only 3-per cent error for k a parts per thousand currency sign 0.2 h Mpc(-1). We use COLA with 10 time steps and a Halo Occupation Distribution to produce 600 mock galaxy catalogues of the WiggleZ Dark Energy Survey. Our parallelized code for efficient generation of accurate halo catalogues is publicly available at https://github.com/junkoda/cola_halo. C1 [Koda, Jun] Osserv Astron Brera, INAF, Via E Bianchi 46, I-23807 Merate, Italy. [Koda, Jun; Blake, Chris; Kazin, Eyal; Marin, Felipe] Swinburne Univ Technol, Ctr Astrophys & Supercomp, POB 218, Hawthorn, Vic 3122, Australia. [Koda, Jun; Kazin, Eyal; Marin, Felipe] ARC Ctr Excellence All Sky Astrophys CAASTRO, Sydney, NSW, Australia. [Beutler, Florian] Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Koda, J (reprint author), Osserv Astron Brera, INAF, Via E Bianchi 46, I-23807 Merate, Italy.; Koda, J (reprint author), Swinburne Univ Technol, Ctr Astrophys & Supercomp, POB 218, Hawthorn, Vic 3122, Australia.; Koda, J (reprint author), ARC Ctr Excellence All Sky Astrophys CAASTRO, Sydney, NSW, Australia. EM jun.koda@brera.inaf.it OI Beutler, Florian/0000-0003-0467-5438 FU Australian Research Council Centre of Excellence for All-sky Astrophysics (CAASTRO) [CE110001020]; European Research Council through the Darklight ERC Advanced Research Grant [291521]; Australian Research Council [FT110100639]; Swinburne; Australian Governments Education Investment Fund FX We thank the anonymous referee for a careful reading of our paper. We thank Svetlin Tassev, Roman Scoccimarro, Volker Springel, and their collaborators for making their codes public; our work was not possible without their public codes. This research was conducted by the Australian Research Council Centre of Excellence for All-sky Astrophysics (CAASTRO), through project number CE110001020. JK also acknowledges support of the European Research Council through the Darklight ERC Advanced Research Grant (#291521). CB acknowledges the support of the Australian Research Council through Future Fellowship awards FT110100639. Our numerical computation was supported by the gSTAR national facility at Swinburne University of Technology, the Flagship Allocation Scheme of the NCI National Facility at the ANU, and the Texas Advanced Computing Center (TACC) at The University of Texas at Austin. gSTAR is funded by Swinburne and the Australian Governments Education Investment Fund. NR 67 TC 6 Z9 6 U1 1 U2 1 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD JUN 21 PY 2016 VL 459 IS 2 BP 2118 EP 2129 DI 10.1093/mnras/stw763 PG 12 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DO0LU UT WOS:000377471200075 ER PT J AU Chai, MF Zhou, CN Molina, I Fu, CX Nakashima, J Li, GF Zhang, WZ Park, JJ Tang, YH Jiang, QZ Wang, ZY AF Chai, Maofeng Zhou, Chuanen Molina, Isabel Fu, Chunxiang Nakashima, Jin Li, Guifen Zhang, Wenzheng Park, Jongjin Tang, Yuhong Jiang, Qingzhen Wang, Zeng-Yu TI A class II KNOX gene, KNOX4, controls seed physical dormancy SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE seed physical dormancy; class II KNOX; hardseededness; Medicago truncatula; seed coat ID LEGUME MEDICAGO-TRUNCATULA; ARABIDOPSIS-THALIANA; CHEMICAL-COMPOSITION; PLANT DEVELOPMENT; HARD-SEEDEDNESS; LIPID POLYESTER; BRASSICA-NAPUS; SOYBEAN SEEDS; CUTICLE; LEAF AB Physical dormancy of seed is an adaptive trait that widely exists in higher plants. This kind of dormancy is caused by a water-impermeable layer that blocks water and oxygen from the surrounding environment and keeps embryos in a viable status for a long time. Most of the work on hardseededness has focused on morphological structure and phenolic content of seed coat. The molecular mechanism underlying physical dormancy remains largely elusive. By screening a large number of Tnt1 retrotransposon-tagged Medicago truncatula lines, we identified nondormant seed mutants from this model legume species. Unlike wild-type hard seeds exhibiting physical dormancy, the mature mutant seeds imbibed water quickly and germinated easily, without the need for scarification. Microscopic observations of cross sections showed that the mutant phenotype was caused by a dysfunctional palisade cuticle layer in the seed coat. Chemical analysis found differences in lipid monomer composition between the wild-type and mutant seed coats. Genetic and molecular analyses revealed that a class II KNOTTED-like homeobox (KNOXII) gene, KNOX4, was responsible for the loss of physical dormancy in the seeds of the mutants. Microarray and chromatin immunoprecipitation analyses identified CYP86A, a gene associated with cutin biosynthesis, as one of the downstream target genes of KNOX4. This study elucidated a novel molecular mechanism of physical dormancy and revealed a new role of class II KNOX genes. Furthermore, KNOX4-like genes exist widely in seed plants but are lacking in nonseed species, indicating that KNOX4 may have diverged from the other KNOXII genes during the evolution of seed plants. C1 [Chai, Maofeng; Zhou, Chuanen; Fu, Chunxiang; Zhang, Wenzheng; Park, Jongjin; Wang, Zeng-Yu] Samuel Roberts Noble Fdn Inc, Forage Improvement Div, Ardmore, OK 73401 USA. [Zhou, Chuanen] Shandong Univ, Sch Life Sci, Jinan 250100, Shandong, Peoples R China. [Molina, Isabel] Algoma Univ, Dept Biol, Sault Ste Marie, ON, Canada. [Fu, Chunxiang] Chinese Acad Sci, Inst BioEnergy & Bioproc Technol, Qingdao 266101, Shandong, Peoples R China. [Nakashima, Jin; Li, Guifen; Tang, Yuhong; Jiang, Qingzhen] Samuel Roberts Noble Fdn Inc, Plant Biol Div, Ardmore, OK 73401 USA. [Park, Jongjin] Oak Ridge Natl Lab, BioEnergy Sci Ctr, Oak Ridge, TN 37831 USA. RP Wang, ZY (reprint author), Samuel Roberts Noble Fdn Inc, Forage Improvement Div, Ardmore, OK 73401 USA. EM zywang@noble.org FU Samuel Roberts Noble Foundation; BioEnergy Science Center; Office of Biological and Environmental Research in the Department of Energy Office of Science FX We thank Amy Mason and Courtney Leeper for critical reading of the manuscript; Dr. Kirankumar Mysore for providing the Tnt1 mutants; Xiaofei Cheng, Kuihua Zhang, and Jiangqi Wen for assistance with screening the Tnt1 mutants; and the greenhouse staff for assistance with plant growth. This work was supported by The Samuel Roberts Noble Foundation and the BioEnergy Science Center. The BioEnergy Science Center is a US Department of Energy Bioenergy Research Center supported by the Office of Biological and Environmental Research in the Department of Energy Office of Science. NR 44 TC 1 Z9 1 U1 15 U2 33 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JUN 21 PY 2016 VL 113 IS 25 BP 6997 EP 7002 DI 10.1073/pnas.1601256113 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DP1TN UT WOS:000378272400057 PM 27274062 ER PT J AU Rakhman, A Hafez, M Nanda, S Benmokhtar, F Camsonne, A Cates, GD Dalton, MM Franklin, GB Friend, M Michaels, RW Nelyubin, V Parno, DS Paschke, KD Quinn, BP Souder, PA Tobias, WA AF Rakhman, A. Hafez, M. Nanda, S. Benmokhtar, F. Camsonne, A. Cates, G. D. Dalton, M. M. Franklin, G. B. Friend, M. Michaels, R. W. Nelyubin, V. Parno, D. S. Paschke, K. D. Quinn, B. P. Souder, P. A. Tobias, W. A. TI A high-finesse Fabry-Perot cavity with a frequency-doubled green laser for precision Compton polarimetry at Jefferson Lab SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Compton polarimetry; Fabry-Perot cavity; Laser polarization; Polarized electron beam ID ELECTRON-BEAM POLARIZATION; BACKSCATTERING POLARIMETER; BIREFRINGENCE; SCATTERING; CALCULUS; LOSSES; JLAB AB A high-finesse Fabry-Perot cavity with a frequency-doubled continuous wave green laser (532 nm) has been built and installed in Hall A of Jefferson Lab for high precision Compton polarimetry. The infrared (1064 nm) beam from a ytterbium-doped fiber amplifier seeded by a Nd:YAG nonplanar ring oscillator laser is frequency doubled in a single-pass periodically poled MgO:LiNbO3 crystal. The maximum achieved green power at 5 W infrared pump power is 1.74 W with a total conversion efficiency of 34.8%. The green beam is injected into the optical resonant cavity and enhanced up to 3.7 kW with a corresponding enhancement of 3800. The polarization transfer function has been measured in order to determine the intra-cavity circular laser polarization within a measurement uncertainty of 0.7%. The PREx experiment at Jefferson Lab used this system for the first time and achieved 1.0% precision in polarization measurements of an electron beam with energy and current of 1.06 GeV and 50 mu A. (C) 2016 Elsevier B.V. All rights reserved. C1 [Rakhman, A.; Souder, P. A.] Syracuse Univ, Dept Phys, Syracuse, NY 13244 USA. [Rakhman, A.] Oak Ridge Natl Lab, Res Accelerator Div, Spallat Neutron Source, Oak Ridge, TN 37831 USA. [Hafez, M.] Old Dominion Univ, Appl Res Ctr, Norfolk, VA 23529 USA. [Nanda, S.; Camsonne, A.; Dalton, M. M.; Michaels, R. W.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. [Benmokhtar, F.; Franklin, G. B.; Friend, M.; Parno, D. S.; Quinn, B. P.] Carnegie Mellon Univ, Dept Phys, Pittsburgh, PA 15213 USA. [Benmokhtar, F.] Duquesne Univ, Pittsburgh, PA 15282 USA. [Cates, G. D.; Dalton, M. M.; Nelyubin, V.; Paschke, K. D.; Tobias, W. A.] Univ Virginia, Dept Phys, Charlottesville, VA 22904 USA. [Friend, M.] High Energy Accelerator Res Org KEK, Tsukuba, Ibaraki, Japan. [Parno, D. S.] Univ Washington, Ctr Expt Nucl Phys & Astrophys, Seattle, WA 98195 USA. [Parno, D. S.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. RP Rakhman, A (reprint author), Oak Ridge Natl Lab, Res Accelerator Div, Spallat Neutron Source, Oak Ridge, TN 37831 USA. EM rahim@ornl.gov RI Franklin, Gregg/N-7743-2014; Quinn, Brian/N-7343-2014; Parno, Diana/B-7546-2017 OI Franklin, Gregg/0000-0003-4176-1378; Quinn, Brian/0000-0003-2800-986X; Parno, Diana/0000-0002-9363-0401 FU DOE [DE-AC05-06OR23177]; Jefferson Science Associates, LLC [DE-FG02-84ER40146] FX The authors wish to thank the Hall A technical staff for their assistance in installing the upgraded system and the JLab Accelerator Division for their efforts to achieve and maintain the high electron beam quality necessary for running the Compton polarimeter. This work is supported by DOE Grants DE-AC05-06OR23177, under which Jefferson Science Associates, LLC, operate Jefferson Lab, and DE-FG02-84ER40146. NR 52 TC 0 Z9 0 U1 1 U2 11 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JUN 21 PY 2016 VL 822 BP 82 EP 96 DI 10.1016/j.nima.2016.03.085 PG 15 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DK1GQ UT WOS:000374660900012 ER PT J AU Qian, ZY Hui, Y Liu, FZ Kang, SH Kar, S Rinaldi, M AF Qian, Zhenyun Hui, Yu Liu, Fangze Kang, Sungho Kar, Swastik Rinaldi, Matteo TI Graphene-aluminum nitride NEMS resonant infrared detector SO MICROSYSTEMS & NANOENGINEERING LA English DT Article DE aluminum nitride; graphene; infrared detector; MEMS; NEMS; piezoelectric; resonant sensor ID LAMB WAVE RESONATORS; GALLIUM NITRIDE; SYSTEMS; MODE AB The use of micro-/nanoelectromechanical resonators for the room temperature detection of electromagnetic radiation at infrared frequencies has recently been investigated, showing thermal detection capabilities that could potentially outperform conventional microbolometers. The scaling of the device thickness in the nanometer range and the achievement of high infrared absorption in such a subwavelength thickness, without sacrificing the electromechanical performance, are the two key challenges for the implementation of fast, high-resolution micro-/nanoelectromechanical resonant infrared detectors. In this paper, we show that by using a virtually massless, high-electrical-conductivity, and transparent graphene electrode, floating at the van der Waals separation of a few angstroms from a piezoelectric aluminum nitride nanoplate, it is possible to implement ultrathin (460 nm) piezoelectric nanomechanical resonant structures with improved electromechanical performance (>50% improved frequency x quality factor) and infrared detection capabilities (>100 x improved infrared absorptance) compared with metal-electrode counterparts, despite their reduced volumes. The intrinsic infrared absorption capabilities of a submicron thin graphene-aluminum nitride plate backed with a metal electrode are investigated for the first time and exploited for the first experimental demonstration of a piezoelectric nanoelectromechanical resonant thermal detector with enhanced infrared absorptance in a reduced volume. Moreover, the combination of electromagnetic and piezoelectric resonances provided by the same graphene-aluminum nitride-metal stack allows the proposed device to selectively detect short-wavelength infrared radiation (by tailoring the thickness of aluminum nitride) with unprecedented electromechanical performance and thermal capabilities. These attributes potentially lead to the development of uncooled infrared detectors suitable for the implementation of high performance, miniaturized and power-efficient multispectral infrared imaging systems. C1 [Qian, Zhenyun; Hui, Yu; Kang, Sungho; Rinaldi, Matteo] Northeastern Univ, Dept Elect & Comp Engn, Boston, MA 02115 USA. [Liu, Fangze; Kar, Swastik] Northeastern Univ, Dept Phys, Boston, MA 02115 USA. [Liu, Fangze] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Rinaldi, M (reprint author), Northeastern Univ, Dept Elect & Comp Engn, Boston, MA 02115 USA. EM rinaldi@ece.neu.edu FU DARPA Young Faculty Award [N66001-12-1-4221]; NSF CAREER Award [ECCS-1350114, ECCS-1351424]; DARPA MTO under the RF-FPGA Program [N66001-14-1-4011]; U.S. Department of Homeland Security, Science and Technology Directorate, Office of University Programs [2013-ST-061-ED0001]; Northeastern University Tier-1 seed grant FX We thank Dr. Mark F. Witinski from Pendar Technologies for providing the QCL prototype and the staff of the George J. Kostas Nanoscale Technology and Manufacturing Research Canter at Northeastern University, where the devices were fabricated. This work was partially supported by the DARPA Young Faculty Award (N66001-12-1-4221), the NSF CAREER Award (ECCS-1350114), DARPA MTO (N66001-14-1-4011) under the RF-FPGA Program, the NSF CAREER Award (ECCS-1351424), the U.S. Department of Homeland Security, Science and Technology Directorate, Office of University Programs, under Grant Award 2013-ST-061-ED0001, and a Northeastern University Tier-1 seed grant. NR 37 TC 1 Z9 1 U1 1 U2 1 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2055-7434 J9 MICROSYST NANOENG JI Microsyst. Nanoeng. PD JUN 20 PY 2016 VL 2 AR UNSP 16026 DI 10.1038/micronano.2016.26 PG 7 WC Instruments & Instrumentation SC Instruments & Instrumentation GA EL9MC UT WOS:000394943400001 ER PT J AU Favart, L Guidal, M Horn, T Kroll, P AF Favart, L. Guidal, M. Horn, T. Kroll, P. TI Deeply virtual meson production on the nucleon SO EUROPEAN PHYSICAL JOURNAL A LA English DT Review ID GENERALIZED PARTON DISTRIBUTIONS; HARD EXCLUSIVE ELECTROPRODUCTION; PION FORM-FACTOR; LIGHT VECTOR-MESONS; J/PSI MESONS; DIFFRACTIVE ELECTROPRODUCTION; RESONANCE REGION; COINCIDENCE MEASUREMENTS; COMPTON-SCATTERING; HADRON STRUCTURE AB We review the status of the data and phenomenology in the generalized parton distribution approach of deep virtual meson production. C1 [Favart, L.] Univ Libre Bruxelles, IIHE CP 230, B-1050 Brussels, Belgium. [Guidal, M.] Univ Paris Saclay, CNRS, IN2P3, Inst Phys Nucl Orsay, F-91406 Orsay, France. [Horn, T.] Catholic Univ Amer, Washington, DC 20064 USA. [Horn, T.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. [Kroll, P.] Univ Wuppertal, Fachbereich Phys, D-42097 Wuppertal, Germany. RP Guidal, M (reprint author), Univ Paris Saclay, CNRS, IN2P3, Inst Phys Nucl Orsay, F-91406 Orsay, France. EM guidal@ipno.in2p3.fr FU "Fonds de la Recherche Scientifique-FNRS" of Belgium; NSF [PHY-1306227]; [ANR-12-MONU-0008-01] FX We are very thankful to A. Borissov, S. Goloskokov, X. Janssen, R. McNulty for the help they kindly provided. LF is supported by the "Fonds de la Recherche Scientifique-FNRS" of Belgium. MG benefitted from the ANR-12-MONU-0008-01 "PARTONS" contract support. TH is supported in part by NSF grant PHY-1306227. NR 112 TC 8 Z9 8 U1 3 U2 3 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6001 EI 1434-601X J9 EUR PHYS J A JI Eur. Phys. J. A PD JUN 20 PY 2016 VL 52 IS 6 AR 158 DI 10.1140/epja/i2016-16158-2 PG 17 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA EA0AX UT WOS:000386247200001 ER PT J AU Kasliwal, MM Cenko, SB Singer, LP Corsi, A Cao, Y Barlow, T Bhalerao, V Bellm, E Cook, D Duggan, GE Ferretti, R Frail, DA Horesh, A Kendrick, R Kulkarni, SR Lunnan, R Palliyaguru, N Laher, R Masci, F Manulis, I Miller, AA Nugent, PE Perley, D Prince, TA Quimby, RM Rana, J Rebbapragada, U Sesar, B Singhal, A Surace, J Van Sistine, A AF Kasliwal, M. M. Cenko, S. B. Singer, L. P. Corsi, A. Cao, Y. Barlow, T. Bhalerao, V. Bellm, E. Cook, D. Duggan, G. E. Ferretti, R. Frail, D. A. Horesh, A. Kendrick, R. Kulkarni, S. R. Lunnan, R. Palliyaguru, N. Laher, R. Masci, F. Manulis, I. Miller, A. A. Nugent, P. E. Perley, D. Prince, T. A. Quimby, R. M. Rana, J. Rebbapragada, U. Sesar, B. Singhal, A. Surace, J. Van Sistine, A. TI iPTF SEARCH FOR AN OPTICAL COUNTERPART TO GRAVITATIONAL- WAVE TRANSIENT GW150914 SO ASTROPHYSICAL JOURNAL LETTERS LA English DT Article DE gravitational waves; methods: observational; techniques: spectroscopic; surveys ID ADVANCED LIGO; SUPERLUMINOUS SUPERNOVAE; TELESCOPE; MERGERS; EMISSION; CURVES AB The intermediate Palomar Transient Factory (iPTF) autonomously responded to and promptly tiled the error region of the first gravitational-wave event GW150914 to search for an optical counterpart. Only a small fraction of the total localized region was immediately visible in the northern night sky, due both to Sun-angle and elevation constraints. Here, we report on the transient candidates identified and rapid follow-up undertaken to determine the nature of each candidate. Even in the small area imaged of 126 deg(2), after extensive filtering, eight candidates were deemed worthy of additional follow-up. Within two hours, all eight were spectroscopically classified by the Keck II telescope. Curiously, even though such events are rare, one of our candidates was a superluminous supernova. We obtained radio data with the Jansky Very Large Array and X-ray follow-up with the Swift satellite for this transient. None of our candidates appear to be associated with the gravitational-wave trigger, which is unsurprising given that GW150914 came from the merger of two stellar-mass black holes. This end-to-end discovery and follow-up campaign bodes well for future searches in this post-detection era of gravitational waves. C1 [Kasliwal, M. M.; Cao, Y.; Barlow, T.; Bellm, E.; Cook, D.; Duggan, G. E.; Kulkarni, S. R.; Lunnan, R.; Miller, A. A.; Prince, T. A.] CALTECH, Cahill Ctr Astrophys, Pasadena, CA 91125 USA. [Cenko, S. B.; Singer, L. P.; Miller, A. A.] NASA, Goddard Space Flight Ctr, Astrophys Sci Div, Greenbelt, MD 20771 USA. [Cenko, S. B.] Univ Maryland, Joint Space Sci Inst, College Pk, MD 20742 USA. [Corsi, A.; Palliyaguru, N.] Texas Tech Univ, Dept Phys, Lubbock, TX 79409 USA. [Bhalerao, V.; Rana, J.; Singhal, A.] IUCAA, Post Bag 4, Pune 411007, Maharashtra, India. [Ferretti, R.] Stockholm Univ, Dept Phys, Oskar Klein Ctr, SE-10691 Stockholm, Sweden. [Frail, D. A.] Natl Radio Astron Observ, Socorro, NM 87801 USA. [Horesh, A.; Manulis, I.] Weizmann Inst Sci, Dept Particle Phys & Astrophys, IL-76100 Rehovot, Israel. [Kendrick, R.] Lockheed Martin Space Syst Co, Palo Alto, CA USA. [Laher, R.; Surace, J.] CALTECH, Spitzer Sci Ctr, M-S 314-6, Pasadena, CA 91125 USA. [Masci, F.] CALTECH, Infrared Proc & Anal Ctr, Pasadena, CA 91125 USA. [Miller, A. A.; Rebbapragada, U.] CALTECH, Jet Prop Lab, 4800 Oak Grove Dr, Pasadena, CA 91109 USA. [Nugent, P. E.] Univ Calif Berkeley, Dept Astron, 601 Campbell Hall, Berkeley, CA 94720 USA. [Nugent, P. E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd,MS 50B-4206, Berkeley, CA 94720 USA. [Perley, D.] Niels Bohr Inst, Dark Cosmol Ctr, Juliane Manes Vej 30, DK-2100 Copenhagen, Denmark. [Quimby, R. M.] San Diego State Univ, San Diego, CA 92182 USA. [Quimby, R. M.] Univ Tokyo, UTIAS, Kavli IPMU WPI, Kashiwa, Chiba 2778583, Japan. [Sesar, B.] Max Planck Inst Astron, Konigstuhl 17, D-69117 Heidelberg, Germany. [Van Sistine, A.] Univ Wisconsin, Dept Phys, Milwaukee, WI 53201 USA. RP Kasliwal, MM (reprint author), CALTECH, Cahill Ctr Astrophys, Pasadena, CA 91125 USA. RI Horesh, Assaf/O-9873-2016; OI Horesh, Assaf/0000-0002-5936-1156; Bhalerao, Varun/0000-0002-6112-7609; Singer, Leo/0000-0001-9898-5597 FU National Science Foundation PIRE program [1545949]; Hubble Fellowship [HST-HF-51325.01]; DOE [DE-AC02-05CH11231]; NSF [1455090] FX Based on observations obtained with the Samuel Oschin Telescope 48 inch and the 60 inch Telescope at the Palomar Observatory as part of the iPTF project, a scientific collaboration among the California Institute of Technology, Los Alamos National Laboratory, the University of Wisconsin-Milwaukee, the Oskar Klein Center, the Weizmann Institute of Science, the TANGO Program of the University System of Taiwan, and the Kavli Institute for the Physics and Mathematics of the universe. M.M.K., R.L., and Y.C. acknowledge support from the National Science Foundation PIRE program grant 1545949. A.A.M. acknowledges support from the Hubble Fellowship HST-HF-51325.01. P.E.N. and Y.C. acknowledge support from the DOE under grant DE-AC02-05CH11231, Analytical Modeling for Extreme-Scale Computing Environments. The National Radio Astronomy Observatory is a facility of the National Science Foundation operated under cooperative agreement by Associated Universities, Inc. A.C. and N.P. acknowledge support from NSF CAREER award 1455090. Part of the research was carried out at the Jet Propulsion Laboratory, California Institute of Technology, under a contract with NASA. M.M.K. thanks Brian Metzger for providing us theoretical light curves for neutron-powered precursors. We thank the referee for constructive feedback. NR 41 TC 7 Z9 7 U1 0 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 2041-8205 EI 2041-8213 J9 ASTROPHYS J LETT JI Astrophys. J. Lett. PD JUN 20 PY 2016 VL 824 IS 2 AR L24 DI 10.3847/2041-8205/824/2/L24 PG 9 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DP0GU UT WOS:000378168200008 ER PT J AU Aartsen, MG Abraham, K Ackermann, M Adams, J Aguilar, JA Ahlers, M Ahrens, M Altmann, D Anderson, T Ansseau, I Anton, G Archinger, M Arguelles, C Arlen, TC Auffenberg, J Bai, X Barwick, SW Baum, V Bay, R Beatty, JJ Tjus, JB Becker, KH Beiser, E BenZvi, S Berghaus, P Berley, D Bernardini, E Bernhard, A Besson, DZ Binder, G Bindig, D Bissok, M Blaufuss, E Blumenthal, J Boersma, DJ Bohm, C Borner, M Bos, F Bose, D Boser, S Botner, O Braun, J Brayeur, L Bretz, HP Buzinsky, N Casey, J Casier, M Cheung, E Chirkin, D Christov, A Clark, K Classen, L Coenders, S Collin, GH Conrad, JM Cowen, DF Silva, AHC Daughhetee, J Davis, JC Day, M de Andre, JPAM De Clercq, C Rosendo, ED Dembinski, H De Ridder, S Desiati, P de Vries, KD de Wasseige, G de With, M DeYoung, T Diaz-Velez, JC di Lorenzo, V Dujmovic, H Dumm, JP Dunkman, M Eberhardt, B Ehrhardt, T Eichmann, B Euler, S Evenson, PA Fahey, S Fazely, AR Feintzeig, J Felde, J Filimonov, K Finley, C Flis, S Fosig, CC Fuchs, T Gaisser, TK Gaior, R Gallagher, J Gerhardt, L Ghorbani, K Gier, D Gladstone, L Glagla, M Glusenkamp, T Goldschmidt, A Golup, G Gonzalez, JG Gora, D Grant, D Griffith, Z Ha, C Haack, C Ismail, AH Hallgren, A Halzen, F Hansen, E Hansmann, B Hansmann, T Hanson, K Hebecker, D Heereman, D Helbing, K Hellauer, R Hickford, S Hignight, J Hill, GC Hoffman, KD Hoffmann, R Holzapfel, K Homeier, A Hoshina, K Huang, F Huber, M Huelsnitz, W Hulth, PO Hultqvist, K In, S Ishihara, A Jacobi, E Japaridze, GS Jeong, M Jero, K Jones, BJP Jurkovic, M Kappes, A Karg, T Karle, A Katz, U Kauer, M Keivani, A Kelley, JL Kemp, J Kheirandish, A Kim, M Kintscher, T Kiryluk, J Klein, SR Kohnen, G Koirala, R Kolanoski, H Konietz, R Kopke, L Kopper, C Kopper, S Koskinen, DJ Kowalski, M Krings, K Kroll, G Kroll, M Kruckl, G Kunnen, J Kunwar, S Kurahashi, N Kuwabara, T Labare, M Lanfranchi, JL Larson, MJ Lennarz, D Lesiak-Bzdak, M Leuermann, M Leuner, J Lu, L Lunemann, J Madsen, J Maggi, G Mahn, KBM Mandelartz, M Maruyama, R Mase, K Matis, HS Maunu, R McNally, F Meagher, K Medici, M Meier, M Meli, A Menne, T Merino, G Meures, T Miarecki, S Middell, E Mohrmann, L Montaruli, T Morse, R Nahnhauer, R Naumann, U Neer, G Niederhausen, H Nowicki, SC Nygren, DR Pollmann, AO Olivas, A Omairat, A O'Murchadha, A Palczewski, T Pandya, H Pankova, DV Paul, L Pepper, JA de los Heros, CP Pfendner, C Pieloth, D Pinat, E Posselt, J Price, PB Przybylski, GT Quinnan, M Raab, C Radel, L Rameez, M Rawlins, K Reimann, R Relich, M Resconi, E Rhode, W Richman, M Richter, S Riedel, B Robertson, S Rongen, M Rott, C Ruhe, T Ryckbosch, D Sabbatini, L Sander, HG Sandrock, A Sandroos, J Sarkar, S Schatto, K Schimp, M Schlunder, P Schmidt, T Schoenen, S Schoneberg, S Schonwald, A Schumacher, L Seckel, D Seunarine, S Soldin, D Song, M Spiczak, GM Spiering, C Stahlberg, M Stamatikos, M Stanev, T Stasik, A Steuer, A Stezelberger, T Stokstad, RG Stossl, A Strom, R Strotjohann, NL Sullivan, GW Sutherland, M Taavola, H Taboada, I Tatar, J Ter-Antonyan, S Terliuk, A Tesic, G Tilav, S Toale, PA Tobin, MN Toscano, S Tosi, D Tselengidou, M Turcati, A Unger, E Usner, M Vallecorsa, S Vandenbroucke, J van Eijndhoven, N Vanheule, S van Santen, J Veenkamp, J Vehring, M Voge, M Vraeghe, M Walck, C Wallace, A Wallraff, M Wandkowsky, N Weaver, C Wendt, C Westerhoff, S Whelan, BJ Wiebe, K Wiebusch, CH Wille, L Williams, DR Wills, L Wissing, H Wolf, M Wood, TR Woschnagg, K Xu, DL Xu, XW Xu, Y Yanez, JP Yodh, G Yoshida, S Zoll, M AF Aartsen, M. G. Abraham, K. Ackermann, M. Adams, J. Aguilar, J. A. Ahlers, M. Ahrens, M. Altmann, D. Anderson, T. Ansseau, I. Anton, G. Archinger, M. Arguelles, C. Arlen, T. C. Auffenberg, J. Bai, X. Barwick, S. W. Baum, V. Bay, R. Beatty, J. J. Tjus, J. Becker Becker, K. -H. Beiser, E. BenZvi, S. Berghaus, P. Berley, D. Bernardini, E. Bernhard, A. Besson, D. Z. Binder, G. Bindig, D. Bissok, M. Blaufuss, E. Blumenthal, J. Boersma, D. J. Bohm, C. Boerner, M. Bos, F. Bose, D. Boeser, S. Botner, O. Braun, J. Brayeur, L. Bretz, H. -P. Buzinsky, N. Casey, J. Casier, M. Cheung, E. Chirkin, D. Christov, A. Clark, K. Classen, L. Coenders, S. Collin, G. H. Conrad, J. M. Cowen, D. F. Silva, A. H. Cruz Daughhetee, J. Davis, J. C. Day, M. de Andre, J. P. A. M. De Clercq, C. Rosendo, E. del Pino Dembinski, H. De Ridder, S. Desiati, P. de Vries, K. D. de Wasseige, G. de With, M. DeYoung, T. Diaz-Velez, J. C. di Lorenzo, V. Dujmovic, H. Dumm, J. P. Dunkman, M. Eberhardt, B. Ehrhardt, T. Eichmann, B. Euler, S. Evenson, P. A. Fahey, S. Fazely, A. R. Feintzeig, J. Felde, J. Filimonov, K. Finley, C. Flis, S. Foesig, C. -C. Fuchs, T. Gaisser, T. K. Gaior, R. Gallagher, J. Gerhardt, L. Ghorbani, K. Gier, D. Gladstone, L. Glagla, M. Gluesenkamp, T. Goldschmidt, A. Golup, G. Gonzalez, J. G. Gora, D. Grant, D. Griffith, Z. Ha, C. Haack, C. Ismail, A. Haj Hallgren, A. Halzen, F. Hansen, E. Hansmann, B. Hansmann, T. Hanson, K. Hebecker, D. Heereman, D. Helbing, K. Hellauer, R. Hickford, S. Hignight, J. Hill, G. C. Hoffman, K. D. Hoffmann, R. Holzapfel, K. Homeier, A. Hoshina, K. Huang, F. Huber, M. Huelsnitz, W. Hulth, P. O. Hultqvist, K. In, S. Ishihara, A. Jacobi, E. Japaridze, G. S. Jeong, M. Jero, K. Jones, B. J. P. Jurkovic, M. Kappes, A. Karg, T. Karle, A. Katz, U. Kauer, M. Keivani, A. Kelley, J. L. Kemp, J. Kheirandish, A. Kim, M. Kintscher, T. Kiryluk, J. Klein, S. R. Kohnen, G. Koirala, R. Kolanoski, H. Konietz, R. Koepke, L. Kopper, C. Kopper, S. Koskinen, D. J. Kowalski, M. Krings, K. Kroll, G. Kroll, M. Krueckl, G. Kunnen, J. Kunwar, S. Kurahashi, N. Kuwabara, T. Labare, M. Lanfranchi, J. L. Larson, M. J. Lennarz, D. Lesiak-Bzdak, M. Leuermann, M. Leuner, J. Lu, L. Lunemann, J. Madsen, J. Maggi, G. Mahn, K. B. M. Mandelartz, M. Maruyama, R. Mase, K. Matis, H. S. Maunu, R. McNally, F. Meagher, K. Medici, M. Meier, M. Meli, A. Menne, T. Merino, G. Meures, T. Miarecki, S. Middell, E. Mohrmann, L. Montaruli, T. Morse, R. Nahnhauer, R. Naumann, U. Neer, G. Niederhausen, H. Nowicki, S. C. Nygren, D. R. Pollmann, A. Obertacke Olivas, A. Omairat, A. O'Murchadha, A. Palczewski, T. Pandya, H. Pankova, D. V. Paul, L. Pepper, J. A. de los Heros, C. Perez Pfendner, C. Pieloth, D. Pinat, E. Posselt, J. Price, P. B. Przybylski, G. T. Quinnan, M. Raab, C. Raedel, L. Rameez, M. Rawlins, K. Reimann, R. Relich, M. Resconi, E. Rhode, W. Richman, M. Richter, S. Riedel, B. Robertson, S. Rongen, M. Rott, C. Ruhe, T. Ryckbosch, D. Sabbatini, L. Sander, H. -G. Sandrock, A. Sandroos, J. Sarkar, S. Schatto, K. Schimp, M. Schlunder, P. Schmidt, T. Schoenen, S. Schoeneberg, S. Schoenwald, A. Schumacher, L. Seckel, D. Seunarine, S. Soldin, D. Song, M. Spiczak, G. M. Spiering, C. Stahlberg, M. Stamatikos, M. Stanev, T. Stasik, A. Steuer, A. Stezelberger, T. Stokstad, R. G. Stoessl, A. Strom, R. Strotjohann, N. L. Sullivan, G. W. Sutherland, M. Taavola, H. Taboada, I. Tatar, J. Ter-Antonyan, S. Terliuk, A. Tesic, G. Tilav, S. Toale, P. A. Tobin, M. N. Toscano, S. Tosi, D. Tselengidou, M. Turcati, A. Unger, E. Usner, M. Vallecorsa, S. Vandenbroucke, J. van Eijndhoven, N. Vanheule, S. van Santen, J. Veenkamp, J. Vehring, M. Voge, M. Vraeghe, M. Walck, C. Wallace, A. Wallraff, M. Wandkowsky, N. Weaver, Ch. Wendt, C. Westerhoff, S. Whelan, B. J. Wiebe, K. Wiebusch, C. H. Wille, L. Williams, D. R. Wills, L. Wissing, H. Wolf, M. Wood, T. R. Woschnagg, K. Xu, D. L. Xu, X. W. Xu, Y. Yanez, J. P. Yodh, G. Yoshida, S. Zoll, M. CA IceCube Collaboration TI AN ALL-SKY SEARCH FOR THREE FLAVORS OF NEUTRINOS FROM GAMMA-RAY BURSTS WITH THE ICECUBE NEUTRINO OBSERVATORY SO ASTROPHYSICAL JOURNAL LA English DT Article DE gamma-ray burst: general; methods: data analysis; neutrinos; telescopes ID HIGH-ENERGY NEUTRINOS; COSMIC-RAYS; TRACK RECONSTRUCTION; SPECTRAL CATALOG; MUON NEUTRINOS; TELESCOPE; ACCELERATION; EMISSION; PERFORMANCE; AMANDA AB We present the results and methodology of a search for neutrinos produced in the decay of charged pions created in interactions between protons and gamma-rays during the prompt emission of 807 gamma-ray bursts (GRBs) over the entire sky. This three-year search is the first in IceCube for shower-like Cherenkov light patterns from electron, muon, and tau neutrinos correlated with GRBs. We detect five low-significance events correlated with five GRBs. These events are consistent with the background expectation from atmospheric muons and neutrinos. The results of this search in combination with those of IceCube's four years of searches for track-like Cherenkov light patterns from muon neutrinos correlated with Northern-Hemisphere GRBs produce limits that tightly constrain current models of neutrino and ultra high energy cosmic ray production in GRB fireballs. C1 [Aartsen, M. G.; Hill, G. C.; Robertson, S.; Wallace, A.; Whelan, B. J.] Univ Adelaide, Dept Phys, Adelaide, SA 5005, Australia. [Abraham, K.; Bernhard, A.; Coenders, S.; Holzapfel, K.; Huber, M.; Jurkovic, M.; Krings, K.; Resconi, E.; Turcati, A.; Veenkamp, J.] Tech Univ Munich, D-85748 Garching, Germany. [Ackermann, M.; Berghaus, P.; Bernardini, E.; Bretz, H. -P.; Silva, A. H. Cruz; Gluesenkamp, T.; Gora, D.; Jacobi, E.; Karg, T.; Kintscher, T.; Kowalski, M.; Kunwar, S.; Middell, E.; Mohrmann, L.; Nahnhauer, R.; Schoenwald, A.; Spiering, C.; Stasik, A.; Stoessl, A.; Strotjohann, N. L.; Terliuk, A.; Usner, M.; van Santen, J.; Yanez, J. P.] DESY, D-15735 Zeuthen, Germany. [Adams, J.] Univ Canterbury, Dept Phys & Astron, Private Bag 4800, Christchurch, New Zealand. [Aguilar, J. A.; Ansseau, I.; Heereman, D.; Meagher, K.; Meures, T.; O'Murchadha, A.; Pinat, E.; Raab, C.] Univ Libre Bruxelles, Sci Fac CP230, B-1050 Brussels, Belgium. [Ahlers, M.; Beiser, E.; Braun, J.; Chirkin, D.; Day, M.; Desiati, P.; Diaz-Velez, J. C.; Fahey, S.; Feintzeig, J.; Ghorbani, K.; Gladstone, L.; Griffith, Z.; Halzen, F.; Hanson, K.; Hoshina, K.; Jero, K.; Karle, A.; Kauer, M.; Kelley, J. L.; Kheirandish, A.; McNally, F.; Merino, G.; Morse, R.; Richter, S.; Sabbatini, L.; Tobin, M. N.; Tosi, D.; Vandenbroucke, J.; Wandkowsky, N.; Wendt, C.; Westerhoff, S.; Wille, L.; Xu, D. L.] Univ Wisconsin, Dept Phys, 1150 Univ Ave, Madison, WI 53706 USA. [Ahlers, M.; Beiser, E.; Braun, J.; Chirkin, D.; Day, M.; Desiati, P.; Diaz-Velez, J. 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R.; Ter-Antonyan, S.; Xu, X. W.] Southern Univ, Dept Phys, Baton Rouge, LA 70813 USA. [Gaior, R.; Ishihara, A.; Kuwabara, T.; Lu, L.; Mase, K.; Relich, M.; Yoshida, S.] Chiba Univ, Dept Phys, Chiba 2638522, Japan. [Gallagher, J.] Univ Wisconsin, Dept Astron, Madison, WI 53706 USA. [Hansen, E.; Koskinen, D. J.; Larson, M. J.; Medici, M.; Sarkar, S.] Univ Copenhagen, Niels Bohr Inst, DK-2100 Copenhagen, Denmark. [Homeier, A.; Voge, M.] Univ Bonn, Inst Phys, D-53115 Bonn, Germany. [Hoshina, K.] Univ Tokyo, Earthquake Res Inst, Bunkyo Ku, Tokyo 1130032, Japan. [Japaridze, G. S.] Clark Atlanta Univ, CTSPS, Atlanta, GA 30314 USA. [Kauer, M.; Maruyama, R.] Yale Univ, Dept Phys, New Haven, CT 06520 USA. [Kiryluk, J.; Lesiak-Bzdak, M.; Niederhausen, H.; Xu, Y.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Kohnen, G.] Univ Mons, B-7000 Mons, Belgium. [Kurahashi, N.; Richman, M.; Wills, L.] Drexel Univ, Dept Phys, 3141 Chestnut St, Philadelphia, PA 19104 USA. [Madsen, J.; Seunarine, S.; Spiczak, G. M.] Univ Wisconsin, Dept Phys, River Falls, WI 54022 USA. [Palczewski, T.; Pepper, J. A.; Toale, P. A.; Williams, D. R.] Univ Alabama, Dept Phys & Astron, Tuscaloosa, AL 35487 USA. [Rawlins, K.] Univ Alaska Anchorage, Dept Phys & Astron, 3211 Providence Dr, Anchorage, AK 99508 USA. [Sarkar, S.] Univ Oxford, Dept Phys, 1 Keble Rd, Oxford OX1 3NP, England. [Stamatikos, M.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. RP Hellauer, R (reprint author), Univ Maryland, Dept Phys, College Pk, MD 20742 USA. EM hellauer@umd.edu RI Anton, Gisela/C-4840-2013; Beatty, James/D-9310-2011; Tjus, Julia/G-8145-2012; Katz, Uli/E-1925-2013; Maruyama, Reina/A-1064-2013; Wiebusch, Christopher/G-6490-2012; Sarkar, Subir/G-5978-2011; Koskinen, David/G-3236-2014; OI Strotjohann, Nora Linn/0000-0002-4667-6730; Anton, Gisela/0000-0003-2039-4724; Beatty, James/0000-0003-0481-4952; Katz, Uli/0000-0002-7063-4418; Maruyama, Reina/0000-0003-2794-512X; Wiebusch, Christopher/0000-0002-6418-3008; Sarkar, Subir/0000-0002-3542-858X; Koskinen, David/0000-0002-0514-5917; Perez de los Heros, Carlos/0000-0002-2084-5866 FU U.S. National Science Foundation-Office of Polar Programs; U.S. National Science Foundation-Physics Division; University of Wisconsin Alumni Research Foundation; Grid Laboratory Of Wisconsin (GLOW) grid infrastructure at the University of Wisconsin-Madison; Open Science Grid (OSG) grid infrastructure; U.S. Department of Energy; National Energy Research Scientific Computing Center; Louisiana Optical Network Initiative (LONI) grid computing resources; Natural Sciences and Engineering Research Council of Canada; WestGrid; Compute/Calcul Canada; Swedish Research Council, Sweden; Swedish Polar Research Secretariat, Sweden; Swedish National Infrastructure for Computing (SNIC), Sweden; Knut and Alice Wallenberg Foundation, Sweden; German Ministry for Education and Research (BMBF), Germany; Deutsche Forschungsgemeinschaft (DFG), Germany; Helmholtz Alliance for Astroparticle Physics (HAP), Germany; Research Department of Plasmas with Complex Interactions (Bochum), Germany; Fund for Scientific Research (FNRS-FWO); FWO Odysseus programme; Flanders Institute to encourage scientific and technological research in industry (IWT); Belgian Federal Science Policy Office (Belspo); University of Oxford, United Kingdom; Marsden Fund, New Zealand; Australian Research Council; Japan Society for Promotion of Science (JSPS); Swiss National Science Foundation (SNSF), Switzerland; National Research Foundation of Korea (NRF); Danish National Research Foundation, Denmark (DNRF) FX We acknowledge the support from the following agencies: the U.S. National Science Foundation-Office of Polar Programs, the U.S. National Science Foundation-Physics Division, the University of Wisconsin Alumni Research Foundation, the Grid Laboratory Of Wisconsin (GLOW) grid infrastructure at the University of Wisconsin-Madison, the Open Science Grid (OSG) grid infrastructure; the U.S. Department of Energy, and the National Energy Research Scientific Computing Center, the Louisiana Optical Network Initiative (LONI) grid computing resources; the Natural Sciences and Engineering Research Council of Canada, WestGrid and Compute/Calcul Canada; the Swedish Research Council, the Swedish Polar Research Secretariat, the Swedish National Infrastructure for Computing (SNIC), and the Knut and Alice Wallenberg Foundation, Sweden; the German Ministry for Education and Research (BMBF), Deutsche Forschungsgemeinschaft (DFG), the Helmholtz Alliance for Astroparticle Physics (HAP), the Research Department of Plasmas with Complex Interactions (Bochum), Germany; the Fund for Scientific Research (FNRS-FWO), the FWO Odysseus programme, Flanders Institute to encourage scientific and technological research in industry (IWT), the Belgian Federal Science Policy Office (Belspo); University of Oxford, United Kingdom; the Marsden Fund, New Zealand; the Australian Research Council; the Japan Society for Promotion of Science (JSPS); the Swiss National Science Foundation (SNSF), Switzerland; the National Research Foundation of Korea (NRF); and the Danish National Research Foundation, Denmark (DNRF). NR 77 TC 4 Z9 4 U1 2 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUN 20 PY 2016 VL 824 IS 2 AR 115 DI 10.3847/0004-637X/824/2/115 PG 13 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DU0RS UT WOS:000381912800051 ER PT J AU Cote, B Ritter, C O'Shea, BW Herwig, F Pignatari, M Jones, S Fryer, CL AF Cote, Benoit Ritter, Christian O'Shea, Brian W. Herwig, Falk Pignatari, Marco Jones, Samuel Fryer, Chris L. CA NuGrid Collaboration TI UNCERTAINTIES IN GALACTIC CHEMICAL EVOLUTION MODELS SO ASTROPHYSICAL JOURNAL LA English DT Article DE Galaxy: abundances; Galaxy: evolution; stars: abundances ID INITIAL MASS FUNCTION; DELAY-TIME DISTRIBUTION; IA SUPERNOVA RATE; CORE-COLLAPSE SUPERNOVAE; EARLY-TYPE GALAXIES; METAL-POOR STARS; MILKY-WAY; STELLAR EVOLUTION; COSMOLOGICAL SIMULATIONS; FORMATION HISTORY AB We use a simple one-zone galactic chemical evolution model to quantify the uncertainties generated by the input parameters in numerical predictions for a galaxy with properties similar to those of the Milky Way. We compiled several studies from the literature to gather the current constraints for our simulations regarding the typical value and uncertainty of the following seven basic parameters: the lower and upper mass limits of the stellar initial mass function (IMF), the slope of the high-mass end of the stellar IMF, the slope of the delay-time distribution function of Type Ia supernovae (SNe Ia), the number of SNe Ia per M-circle dot formed, the total stellar mass formed, and the final mass of gas. We derived a probability distribution function to express the range of likely values for every parameter, which were then included in a Monte Carlo code to run several hundred simulations with randomly selected input parameters. This approach enables us to analyze the predicted chemical evolution of 16 elements in a statistical manner by identifying the most probable solutions, along with their 68% and 95% confidence levels. Our results show that the overall uncertainties are shaped by several input parameters that individually contribute at different metallicities, and thus at different galactic ages. The level of uncertainty then depends on the metallicity and is different from one element to another. Among the seven input parameters considered in this work, the slope of the IMF and the number of SNe Ia are currently the two main sources of uncertainty. The thicknesses of the uncertainty bands bounded by the 68% and 95% confidence levels are generally within 0.3 and 0.6 dex, respectively. When looking at the evolution of individual elements as a function of galactic age instead of metallicity, those same thicknesses range from 0.1 to 0.6 dex for the 68% confidence levels and from 0.3 to 1.0 dex for the 95% confidence levels. The uncertainty in our chemical evolution model does not include uncertainties relating to stellar yields, star formation and merger histories, and modeling assumptions. C1 [Cote, Benoit; Ritter, Christian; Herwig, Falk] Univ Victoria, Dept Phys & Astron, POB 3055, Victoria, BC V8W 2Y2, Canada. [Cote, Benoit] Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA. [Cote, Benoit; Ritter, Christian; O'Shea, Brian W.; Herwig, Falk] Joint Inst Nucl Astrophys Ctr Evolut Elements, E Lansing, MI 48824 USA. [O'Shea, Brian W.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [O'Shea, Brian W.] Michigan State Univ, Dept Computat Math Sci & Engn, E Lansing, MI 48824 USA. [Pignatari, Marco] Univ Hull, Dept Math & Phys, EA Milne Ctr Astrophys, Kingston Upon Hull HU6 7RX, N Humberside, England. [Pignatari, Marco] Hungarian Acad Sci, Res Ctr Astron & Earth Sci, Konkoly Observ, Konkoly Thege Miklos Ut 15-17, H-1121 Budapest, Hungary. [Jones, Samuel] Heidelberg Inst Theoret Studies, Schloss Wolfsbrunnenweg 35, D-69118 Heidelberg, Germany. [Fryer, Chris L.] LANL, Computat Phys & Methods CCS 2, Los Alamos, NM 87545 USA. RP Cote, B (reprint author), Univ Victoria, Dept Phys & Astron, POB 3055, Victoria, BC V8W 2Y2, Canada.; Cote, B (reprint author), Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA.; Cote, B (reprint author), Joint Inst Nucl Astrophys Ctr Evolut Elements, E Lansing, MI 48824 USA. OI Cote, Benoit/0000-0002-9986-8816; Pignatari, Marco/0000-0002-9048-6010 FU National Science Foundation (USA) [PHY-1430152]; FRQNT (Quebec, Canada) postdoctoral fellowship program; National Aeronautics and Space Administration (USA) [NNX12AC98G, HST-AR-13261.01-A]; sabbatical visitor program at the Michigan Institute for Research in Astrophysics (MIRA) at the University of Michigan in Ann Arbor; NSERC Discovery grant (Canada); Canarie; Hungarian Academy of Science (Hungary); Swiss National Science Foundation (Switzerland); U.S. Department of Energy; [W-7405-ENG-36] FX This research is supported by the National Science Foundation (USA) under grant No. PHY-1430152 (JINA Center for the Evolution of the Elements), and by the FRQNT (Quebec, Canada) postdoctoral fellowship program. B.W.O. was supported by the National Aeronautics and Space Administration (USA) through grant NNX12AC98G and Hubble Theory grant HST-AR-13261.01-A. He was also supported in part by the sabbatical visitor program at the Michigan Institute for Research in Astrophysics (MIRA) at the University of Michigan in Ann Arbor, and gratefully acknowledges their hospitality. F.H. acknowledges support through an NSERC Discovery grant (Canada). The NuGrid WENDI platform has been developed as part of the CANFAR NEP project Software-as-a-service for Big Data Analysis funded by Canarie. M.P. was supported by the Lendulet-2014 program from the Hungarian Academy of Science (Hungary) and the Swiss National Science Foundation (Switzerland). S.J. is a fellow of the Alexander von Humboldt Foundation. C.F. was funded in part under the auspices of the U.S. Department of Energy, and supported by its contract W-7405-ENG-36 to Los Alamos National Laboratory. NR 183 TC 6 Z9 6 U1 1 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUN 20 PY 2016 VL 824 IS 2 AR 82 DI 10.3847/0004-637X/824/2/82 PG 19 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DU0RS UT WOS:000381912800018 ER PT J AU De Rosa, RJ Rameau, J Patience, J Graham, JR Doyon, R Lafreniere, D Macintosh, B Pueyo, L Rajan, A Wang, JJ Ward-Duong, K Hung, LW Maire, J Nielsen, EL Ammons, SM Bulger, J Cardwell, A Chilcote, JK Galvez, RL Gerard, BL Goodsell, S Hartung, M Hibon, P Ingraham, P Johnson-Groh, M Kalas, P Konopacky, QM Marchis, F Marois, C Metchev, S Morzinski, KM Oppenheimer, R Perrin, MD Rantakyro, FT Savransky, D Thomas, S AF De Rosa, Robert J. Rameau, Julien Patience, Jenny Graham, James R. Doyon, Rene Lafreniere, David Macintosh, Bruce Pueyo, Laurent Rajan, Abhijith Wang, Jason J. Ward-Duong, Kimberly Hung, Li-Wei Maire, Jerome Nielsen, Eric L. Ammons, S. Mark Bulger, Joanna Cardwell, Andrew Chilcote, Jeffrey K. Galvez, Ramon L. Gerard, Benjamin L. Goodsell, Stephen Hartung, Markus Hibon, Pascale Ingraham, Patrick Johnson-Groh, Mara Kalas, Paul Konopacky, Quinn M. Marchis, Franck Marois, Christian Metchev, Stanimir Morzinski, Katie M. Oppenheimer, Rebecca Perrin, Marshall D. Rantakyro, Fredrik T. Savransky, Dmitry Thomas, Sandrine TI SPECTROSCOPIC CHARACTERIZATION OF HD 95086 b WITH THE GEMINI PLANET IMAGER SO ASTROPHYSICAL JOURNAL LA English DT Article DE infrared: planetary systems; instrumentation: adaptive optics; planets and satellites: atmospheres stars; individual (HD 95086) ID HR 8799 PLANETS; LOW-MASS STARS; EXTRASOLAR GIANT PLANETS; HUBBLE-SPACE-TELESCOPE; INFRARED FILTER SET; YOUNG SOLAR ANALOG; BETA-PICTORIS B; VERY-LOW-MASS; BROWN DWARFS; T-DWARF AB We present new H (1.51.8 mu m) photometric and K-1 (1.92.2 mu m) spectroscopic observations of the young exoplanet HD 95086 b obtained with the Gemini Planet Imager. The Hband magnitude has been significantly improved relative to previous measurements, whereas the lowresolution K-1 (lambda/delta lambda approximate to 66) spectrum is featureless within the measurement uncertainties and presents a monotonically increasing pseudocontinuum consistent with a cloudy atmosphere. By combining these new measurements with literature L' photometry, we compare the spectral energy distribution (SED) of the planet to other young planetarymass companions, field brown dwarfs, and to the predictions of grids of model atmospheres. HD 95086 b is over a magnitude redder in K-1 - L' color than 2MASS J120733463932539 b and HR 8799 c and d, despite having a similar L' magnitude. Considering only the near-infrared measurements, HD 95086 b is most analogous to the brown dwarfs 2MASS J2244316+204343 and 2MASS J21481633+4003594, both of which are thought to have dusty atmospheres. Morphologically, the SED of HD 95086 b is best fit by low temperature (T-eff = 8001300 K), low surface gravity spectra from models which simulate high photospheric dust content. This range of effective temperatures is consistent with field L/T transition objects, but the spectral type of HD 95086 b is poorly constrained between early L and late T due to its unusual position the colormagnitude diagram, demonstrating the difficulty in spectral typing young, low surface gravity substellar objects. As one of the reddest such objects, HD 95086 b represents an important empirical benchmark against which our current understanding of the atmospheric properties of young extrasolar planets can be tested. C1 [De Rosa, Robert J.; Graham, James R.; Wang, Jason J.; Kalas, Paul] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. [Rameau, Julien; Doyon, Rene; Lafreniere, David] Univ Montreal, Dept Phys, Inst Rech Exoplanetes, Montreal, PQ H3C 3J7, Canada. [Patience, Jenny; Rajan, Abhijith; Ward-Duong, Kimberly] Arizona State Univ, Sch Earth & Space Explorat, POB 871404, Tempe, AZ 85287 USA. [Macintosh, Bruce; Nielsen, Eric L.] Stanford Univ, Kavli Inst Particle Astrophys & Cosmol, Stanford, CA 94305 USA. [Pueyo, Laurent; Perrin, Marshall D.] Space Telescope Sci Inst, 3700 San Martin Dr, Baltimore, MD 21218 USA. [Hung, Li-Wei] Univ Calif Los Angeles, Dept Phys & Astron, 430 Portola Plaza, Los Angeles, CA 90095 USA. [Maire, Jerome; Chilcote, Jeffrey K.] Univ Toronto, Dunlap Inst Astron & Astrophys, Toronto, ON M5S 3H4, Canada. [Nielsen, Eric L.; Kalas, Paul; Marchis, Franck] Carl Sagan Ctr, SETI Inst, 189 Bernardo Ave, Mountain View, CA 94043 USA. [Ammons, S. Mark] Lawrence Livermore Natl Lab, L-210,7000 East Ave, Livermore, CA 94550 USA. [Bulger, Joanna] NAOJ, Subaru Telescope, 650 North Aohoku Pl, Hilo, HI 96720 USA. [Cardwell, Andrew] Univ Arizona, Large Binocular Telescope Observ, 933 N Cherry Ave, Tucson, AZ 85721 USA. [Galvez, Ramon L.; Hartung, Markus; Rantakyro, Fredrik T.] Gemini Observ, Casilla 603, La Serena, Chile. [Gerard, Benjamin L.; Johnson-Groh, Mara; Marois, Christian; Thomas, Sandrine] Univ Victoria, Dept Phys & Astron, 3800 Finnerty Rd, Victoria, BC V8P 5C2, Canada. [Goodsell, Stephen] Univ Durham, Dept Phys, Stockton Rd, Durham DH1 3LE, England. [Goodsell, Stephen] Gemini Observ, 670 N Aohoku Pl, Hilo, HI 96720 USA. [Hibon, Pascale] European Southern Observ, Alonso Cordova 3107,Casilla 19001, Santiago, Chile. [Ingraham, Patrick] Large Synopt Survey Telescope, 950 N Cherry Ave, Tucson, AZ 85719 USA. [Konopacky, Quinn M.] Univ Calif San Diego, Ctr Astrophys & Space Sci, La Jolla, CA 92093 USA. [Marois, Christian] Natl Res Council Canada Herzberg, 5071 West Saanich Rd, Victoria, BC V9E 2E7, Canada. [Metchev, Stanimir] Univ Western Ontario, Dept Phys & Astron, Ctr Planetary Sci & Explorat, London, ON N6A 3K7, Canada. [Metchev, Stanimir] SUNY Stony Brook, Dept Phys & Astron, 100 Nicolls Rd, Stony Brook, NY 11790 USA. [Morzinski, Katie M.] Univ Arizona, Steward Observ, 933 N Cherry Ave, Tucson, AZ 85721 USA. [Oppenheimer, Rebecca] Amer Museum Nat Hist, New York, NY 10024 USA. [Savransky, Dmitry] Cornell Univ, Sibley Sch Mech & Aerosp Engn, Ithaca, NY 14853 USA. RP De Rosa, RJ (reprint author), Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. RI Savransky, Dmitry/M-1298-2014; OI Savransky, Dmitry/0000-0002-8711-7206; De Rosa, Robert/0000-0002-4918-0247; Nielsen, Eric/0000-0001-6975-9056; Wang, Jason/0000-0003-0774-6502 FU National Aeronautics and Space Administration; National Science Foundation; NSF [AST-1518332, AST-1411868, DGE-1311230]; NASA [NNX15AD95G/NEXSS, NNX15AC89G, NNX14AJ80G]; Fonds de Recherche du Quebec; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX The authors wish to thank Jonathan Gagne for useful discussions regarding empirical comparisons, and the referee for their comments which helped improve the manuscript. This work was based on observations obtained at the Gemini Observatory, which is operated by the Association of Universities for Research in Astronomy, Inc., under a cooperative agreement with the National Science Foundation (NSF) on behalf of the Gemini partnership: the NSF (United States), the National Research Council (Canada), CONICYT (Chile), the Australian Research Council (Australia), Ministerio da Ciencia, Tecnologia e Inovacao (Brazil) and Ministerio de Ciencia, Tecnologia e Innovacion Productiva (Argentina). This research has made use of the SIMBAD database, operated at CDS, Strasbourg, France. This publication makes use of data products from the Two Micron All Sky Survey, which is a joint project of the University of Massachusetts and the Infrared Processing and Analysis Center/California Institute of Technology, funded by the National Aeronautics and Space Administration and the National Science Foundation. This publication makes use of data products from the Wide-field Infrared Survey Explorer, which is a joint project of the University of California, Los Angeles, and the Jet Propulsion Laboratory/California Institute of Technology, and NEOWISE, which is a project of the Jet Propulsion Laboratory/California Institute of Technology. WISE and NEOWISE are funded by the National Aeronautics and Space Administration. Supported by NSF grants AST-1518332 (R.J.D.R., J.R.G., J.J.W., P.K.), AST-1411868 (J.L.P., B.M., A.R.), and DGE-1311230 (K.W.D.). Supported by NASA grants NNX15AD95G/NEXSS and NNX15AC89G (R.J.D.R., J.R.G., J.J.W., P.K.), and NNX14AJ80G (B.M., E.L.N., F.M.). J.R., R.D. and D.L. acknowledge support from the Fonds de Recherche du Quebec. Portions of this work were performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 143 TC 2 Z9 2 U1 1 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUN 20 PY 2016 VL 824 IS 2 AR 121 DI 10.3847/0004-637X/824/2/121 PG 18 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DU0RS UT WOS:000381912800057 ER PT J AU Jee, MJ Tyson, JA Hilbert, S Schneider, MD Schmidt, S Wittman, D AF Jee, M. James Tyson, J. Anthony Hilbert, Stefan Schneider, Michael D. Schmidt, Samuel Wittman, David TI COSMIC SHEAR RESULTS FROM THE DEEP LENS SURVEY. II. FULL COSMOLOGICAL PARAMETER CONSTRAINTS FROM TOMOGRAPHY SO ASTROPHYSICAL JOURNAL LA English DT Article DE cosmological parameters; cosmology: observations; dark matter; gravitational lensing: weak; large-scale structure of universe ID BARYON ACOUSTIC-OSCILLATIONS; INTRINSIC GALAXY ALIGNMENTS; DARK-ENERGY CONSTRAINTS; HUBBLE-SPACE-TELESCOPE; MATTER POWER SPECTRUM; DIGITAL SKY SURVEY; REDSHIFT DISTRIBUTIONS; DATA RELEASE; WEAK; CFHTLENS AB We present a tomographic cosmic shear study from the Deep Lens Survey (DLS), which, providing a limiting magnitude r(lim) similar to 27 (5 sigma), is designed as a precursor Large Synoptic Survey Telescope (LSST) survey with an emphasis on depth. Using five tomographic redshift bins, we study their auto- and cross-correlations to constrain cosmological parameters. We use a luminosity-dependent nonlinear model to account for the astrophysical systematics originating from intrinsic alignments of galaxy shapes. We find that the cosmological leverage of the DLS is among the highest among existing > 10 deg(2) cosmic shear surveys. Combining the DLS tomography with the 9 yr results of the Wilkinson Microwave Anisotropy Probe (WMAP9) gives Omega(m) = 0.293(-0.014)(+0.012), sigma(8) = 0.833(-0.018)(+0.011), H-0 = 68.6(-1.2)(+1.4) km s(-1) Mpc(-1).4 1 1, and Omega(b) = 0.0475 +/- 0.0012 for Lambda CDM, reducing the uncertainties of the WMAP9-only constraints by similar to 50%. When we do not assume flatness for Lambda CDM, we obtain the curvature constraint Omega(k) = -0.010(-0.015)(+0.013) from the DLS+WMAP9 combination, which, however, is not well constrained when WMAP9 is used alone. The dark energy equation-of-state parameter w is tightly constrained when baryonic acoustic oscillation (BAO) data are added, yielding = - w -1.02(-0.09)(+0.10) with the DLS+WMAP9+BAO joint probe. The addition of supernova constraints further tightens the parameter to w = -1.03 +/- 0.03. Our joint constraints are fully consistent with the final Planck results and also with the predictions of a Lambda CDM universe. C1 [Jee, M. James] Yonsei Univ, Dept Astron, 50 Yonsei Ro, Seoul 03722, South Korea. [Jee, M. James] Yonsei Univ, Ctr Galaxy Evolut Res, 50 Yonsei Ro, Seoul 03722, South Korea. [Jee, M. James; Tyson, J. Anthony; Schmidt, Samuel; Wittman, David] Univ Calif Davis, Dept Phys, One Shields Ave, Davis, CA 95616 USA. [Hilbert, Stefan] Excellence Cluster Universe, Boltzmannstr 2, D-85748 Garching, Germany. [Hilbert, Stefan] Univ Munich, Univ Sternwarte, Scheinerstr 1, D-81679 Munich, Germany. [Schneider, Michael D.] Lawrence Livermore Natl Lab, POB 808 L-210, Livermore, CA 94551 USA. RP Jee, MJ (reprint author), Yonsei Univ, Dept Astron, 50 Yonsei Ro, Seoul 03722, South Korea.; Jee, MJ (reprint author), Yonsei Univ, Ctr Galaxy Evolut Res, 50 Yonsei Ro, Seoul 03722, South Korea.; Jee, MJ (reprint author), Univ Calif Davis, Dept Phys, One Shields Ave, Davis, CA 95616 USA. EM mkjee@physics.ucdavis.edu OI Schneider, Michael/0000-0002-8505-7094 FU National Research Foundation of Korea; Yonsei University New Faculty Research Infrastructure Support Program; NSF [AST-1108893, AST-0134753, AST-0441072, AST-0708433, AST-0807458-002]; DOE [DE-FG02-07ER41505, DE-FG02-91ER40674]; Lucent Technologies Bell Laboratories; DFG cluster of excellence "Origin and Structure of the Universe"; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX M.J.J. acknowledges support for the current research from the National Research Foundation of Korea to the Center for Galaxy Evolution Research and from the Yonsei University New Faculty Research Infrastructure Support Program. We thank Perry Gee for carefully managing the DLS database. The development of the StackFit algorithm and its application to the DLS were funded in part by NSF grant AST-1108893 and DOE grants DE-FG02-07ER41505 and DE-FG02-91ER40674. The DLS and our systematics reduction R&D have received major funding from Lucent Technologies Bell Laboratories and from the NSF (grants AST-0134753, AST-0441072, AST-1108893, and AST-0708433). S.H. acknowledges support by NSF grant no. AST-0807458-002 and support by the DFG cluster of excellence "Origin and Structure of the Universe" (www.universe-cluster.de). Part of this work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. This work is based on observations at Kitt Peak National Observatory and Cerro Tololo Inter-American Observatory, which are operated by the Association of Universities for Research in Astronomy (AURA) under a cooperative agreement with the National Science Foundation. NR 82 TC 3 Z9 3 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUN 20 PY 2016 VL 824 IS 2 AR 77 DI 10.3847/0004-637X/824/2/77 PG 19 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DU0RS UT WOS:000381912800013 ER PT J AU Kaurov, AA Gnedin, NY AF Kaurov, Alexander A. Gnedin, Nickolay Y. TI COSMIC REIONIZATION ON COMPUTERS. MEAN AND FLUCTUATING REDSHIFTED 21 cm SIGNAL SO ASTROPHYSICAL JOURNAL LA English DT Article DE cosmology: theory; intergalactic medium; methods: numerical ID SIMILAR-TO 20; POWER SPECTRUM; PAPER-64 CONSTRAINTS; INTERGALACTIC MEDIUM; DARK-AGES; EPOCH; GALAXIES; SIMULATIONS; UNIVERSE; IMPACT AB We explore the mean and fluctuating redshifted 21 cm signal in numerical simulations from the Cosmic Reionization On Computers project. We find that the mean signal varies between about +/- 25 mK. Most significantly, we find that the negative pre-reionization dip at z similar to 10-15 only extends to similar to -25 mK, requiring substantially higher sensitivity from global signal experiments that operate in this redshift range (EDGES-II, LEDA, SCI-HI, and DARE) than has often been assumed previously. We also explore the role of dense substructure (filaments and embedded galaxies) in the formation of the 21 cm power spectrum. We find that by neglecting the semi-neutral substructure inside ionized bubbles, the power spectrum can be misestimated by 25%-50% at scales k similar to 0.1-1h Mpc(-1). This scale range is of particular interest, because the upcoming 21 cm experiments (Murchison Widefield Array, Precision Array for Probing the Epoch of Reionization, Hydrogen Epoch of Reionization Array) are expected to be most sensitive within it. C1 [Kaurov, Alexander A.; Gnedin, Nickolay Y.] Univ Chicago, Dept Astron & Astrophys, Chicago, IL 60637 USA. [Gnedin, Nickolay Y.] Fermilab Natl Accelerator Lab, Ctr Particle Astrophys, Batavia, IL 60510 USA. [Gnedin, Nickolay Y.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Gnedin, Nickolay Y.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. RP Kaurov, AA (reprint author), Univ Chicago, Dept Astron & Astrophys, Chicago, IL 60637 USA. EM kaurov@uchicago.edu; gnedin@fnal.gov FU United States Department of Energy [DE-AC02-07CH11359]; NSF [AST-1211190]; DOE Office of Science User Facility [DE-AC02-06CH11357] FX Fermilab is operated by Fermi Research Alliance, LLC, under Contract No. DE-AC02-07CH11359 with the United States Department of Energy. This work was also supported in part by the NSF grant AST-1211190. Simulations used in this work have been performed on the National Energy Research Supercomputing Center (NERSC) supercomputers "Hopper" and "Edison" and on the Argonne Leadership Computing Facility supercomputer "Mira." An award of computer time was provided by the Innovative and Novel Computational Impact on Theory and Experiment (INCITE) program. This research used resources of the Argonne Leadership Computing Facility, which is a DOE Office of Science User Facility supported under Contract DE-AC02-06CH11357. NR 34 TC 1 Z9 1 U1 2 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUN 20 PY 2016 VL 824 IS 2 AR 114 DI 10.3847/0004-637X/824/2/114 PG 7 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DU0RS UT WOS:000381912800050 ER PT J AU Yukita, M Hornschemeier, AE Lehmer, BD Ptak, A Wik, DR Zezas, A Antoniou, V Maccarone, TJ Replicon, V Tyler, JB Venters, T Argo, MK Bechtol, K Boggs, S Christensen, FE Craig, WW Hailey, C Harrison, F Krivonos, R Kuntz, K Stern, D Zhang, WW AF Yukita, M. Hornschemeier, A. E. Lehmer, B. D. Ptak, A. Wik, D. R. Zezas, A. Antoniou, V. Maccarone, T. J. Replicon, V. Tyler, J. B. Venters, T. Argo, M. K. Bechtol, K. Boggs, S. Christensen, F. E. Craig, W. W. Hailey, C. Harrison, F. Krivonos, R. Kuntz, K. Stern, D. Zhang, W. W. TI A HARD X-RAY STUDY OF THE NORMAL STAR-FORMING GALAXY M83 WITH NuSTAR SO ASTROPHYSICAL JOURNAL LA English DT Article DE galaxies: individual (M83); galaxies: starburst; galaxies: star formation; X-rays: galaxies ID XMM-NEWTON; STARBURST GALAXY; HOST GALAXIES; BROAD-BAND; ULTRALUMINOUS STATE; BINARY POPULATIONS; NUCLEAR STARBURST; FORMATION HISTORY; MAGELLANIC-CLOUD; CENTRAL REGION AB We present the results from sensitive, multi-epoch NuSTAR observations of the late-type star-forming galaxy M83 (d = 4.6 Mpc). This is the first investigation to spatially resolve the hard (E > 10 keV) X-ray emission of this galaxy. The nuclear region and similar to 20 off-nuclear point sources, including a previously discovered ultraluminous X-ray source, are detected in our NuSTAR observations. The X-ray hardnesses and luminosities of the majority of the point sources are consistent with hard X-ray sources resolved in the starburst galaxy NGC 253. We infer that the hard X-ray emission is most likely dominated by intermediate accretion state black hole binaries and neutron star low-mass X-ray binaries (Z-sources). We construct the X-ray binary luminosity function (XLF) in the NuSTAR band for an extragalactic environment for the first time. The M83 XLF has a steeper XLF than the X-ray binary XLF in NGC 253, which is consistent with previous measurements by Chandra at softer X-ray energies. The NuSTAR integrated galaxy spectrum of M83 drops quickly above 10 keV, which is also seen in the starburst galaxies NGC 253, NGC 3310, and NGC 3256. The NuSTAR observations constrain any active galactic nucleus (AGN) to be either highly obscured or to have an extremely low luminosity of less than or similar to 10(38) erg s(-1) (10-30 keV), implying that it is emitting at a very low Eddington ratio. An X-ray point source that is consistent with the location of the nuclear star cluster with an X-ray luminosity of a few times 1038 erg s(-1) may be a low-luminosity AGN but is more consistent with being an X-ray binary. C1 [Yukita, M.; Hornschemeier, A. E.; Lehmer, B. D.; Ptak, A.; Wik, D. R.; Kuntz, K.] Johns Hopkins Univ, Homewood Campus, Baltimore, MD 21218 USA. [Yukita, M.; Hornschemeier, A. E.; Lehmer, B. D.; Ptak, A.; Wik, D. R.; Tyler, J. B.; Venters, T.; Zhang, W. W.] NASA, Goddard Space Flight Ctr, Code 662, Greenbelt, MD 20771 USA. [Lehmer, B. D.] Univ Arkansas, Dept Phys, Fayetteville, AR 72701 USA. [Zezas, A.] Univ Crete, Dept Phys, Iraklion, Greece. [Zezas, A.; Antoniou, V.] Harvard Smithsonian Ctr Astrophys, 60 Garden St, Cambridge, MA 02138 USA. [Maccarone, T. J.] Texas Tech Univ, Dept Phys, Lubbock, TX 79409 USA. [Replicon, V.] New Mexico Inst Min & Technol, Dept Phys, Socorro, NM 87801 USA. [Tyler, J. B.] Catholic Univ Amer, Inst Astrophys & Computat Sci, Dept Phys, Washington, DC 20064 USA. [Argo, M. K.] Univ Manchester, Jodrell Bank, Ctr Astrophys, Oxford Rd, Manchester M13 9PL, Lancs, England. [Bechtol, K.] Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Boggs, S.; Krivonos, R.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Christensen, F. E.] Tech Univ Denmark, Natl Space Inst, DK-2100 Copenhagen, Denmark. [Craig, W. W.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Hailey, C.] Columbia Univ, New York, NY USA. [Harrison, F.] CALTECH, Div Phys Math & Astron, Pasadena, CA 91125 USA. [Krivonos, R.] Russian Acad Sci, Space Res Inst, Profsoyuznaya 84-32, Moscow 117997, Russia. [Stern, D.] CALTECH, Jet Prop Lab, 4800 Oak Grove Dr, Pasadena, CA 91109 USA. RP Yukita, M (reprint author), Johns Hopkins Univ, Homewood Campus, Baltimore, MD 21218 USA.; Yukita, M (reprint author), NASA, Goddard Space Flight Ctr, Code 662, Greenbelt, MD 20771 USA. RI Boggs, Steven/E-4170-2015; Yukita, Mihoko/E-4135-2017; Zezas, Andreas/C-7543-2011; OI Boggs, Steven/0000-0001-9567-4224; Zezas, Andreas/0000-0001-8952-676X; Argo, Megan/0000-0003-3594-0214 FU NASA [NNG08FD60C]; National Aeronautics and Space Administration [GO4-15086Z, NAS8-03060]; Russian Science Foundation [14-12-01315] FX We thank the referee for useful comments and suggests that improved this paper. This work was supported under NASA Contract No. NNG08FD60C, and made use of data from the NuSTAR mission, a project led by the California Institute of Technology, managed by the Jet Propulsion Laboratory, and funded by the National Aeronautics and Space Administration. We sincerely thank Karl Forster and Brian Grefenstette for their work on the complicated stray light pattern and for assistance in designing the NuSTAR observational setup for minimizing this contamination. We also thank NuSTAR and Chandra mission planners for making the Chandra and NuSTAR observations simultaneous. We also thank P. Tzanavaris and D. Swartz for helpful discussion. Support for this work was provided by the National Aeronautics and Space Administration through Chandra Award Number GO4-15086Z issued by the Chandra X-ray Observatory Center, which is operated by the Smithsonian Astrophysical Observatory for and on behalf of the National Aeronautics Space Administration under contract NAS8-03060. R.K. acknowledges support from Russian Science Foundation (grant 14-12-01315). NR 73 TC 0 Z9 0 U1 1 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUN 20 PY 2016 VL 824 IS 2 AR 107 DI 10.3847/0004-637X/824/2/107 PG 23 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DU0RS UT WOS:000381912800043 ER PT J AU Coletta, M McLellan, R Murphy, P Leube, BT Sanz, S Clowes, R Gagnon, KJ Teat, SJ Cooper, AI Paterson, MJ Brechin, EK Dalgarno, SJ AF Coletta, Marco McLellan, Ross Murphy, Paul Leube, Bernhard T. Sanz, Sergio Clowes, Rob Gagnon, Kevin J. Teat, Simon J. Cooper, Andrew I. Paterson, Martin J. Brechin, Euan K. Dalgarno, Scott J. TI Bis-Calix[4]arenes: From Ligand Design to the Directed Assembly of a Metal-Organic Trigonal Antiprism SO CHEMISTRY-A EUROPEAN JOURNAL LA English DT Article DE calixarenes; clusters; directed assembly; gas storage; metal-organic polyhedron ID SINGLE-MOLECULE MAGNETS; BUILDING-BLOCKS; CLUSTER; POLYHEDRA; DENSITY AB Calix[4]arenes (C[4]s) are versatile platforms for the construction of polymetallic clusters containing paramagnetic metal ions. Synthetic modification at the C[4] methylene bridge allows for the design of bis-C[4]s that, depending on the linker employed, can be used to either dictate which clusters can be formed or direct the assembly of a new metal-organic polyhedron (MOP). The assembly resulting from the latter approach displays thermal stability and uptake of N-2 or H-2 gas, confirming that this is a viable route to the synthesis of new, functional supramolecular architectures. C1 [Coletta, Marco; McLellan, Ross; Murphy, Paul; Leube, Bernhard T.; Paterson, Martin J.; Dalgarno, Scott J.] Heriot Watt Univ, Inst Chem Sci, Edinburgh EH14 4AS, Midlothian, Scotland. [Sanz, Sergio; Brechin, Euan K.] Univ Edinburgh, EaStCHEM Sch Chem, David Brewster Rd, Edinburgh EH9 3FJ, Midlothian, Scotland. [Clowes, Rob; Cooper, Andrew I.] Univ Liverpool, Dept Chem, Crown St, Liverpool L69 7ZD, Merseyside, England. [Gagnon, Kevin J.; Teat, Simon J.] Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA USA. RP Dalgarno, SJ (reprint author), Heriot Watt Univ, Inst Chem Sci, Edinburgh EH14 4AS, Midlothian, Scotland.; Brechin, EK (reprint author), Univ Edinburgh, EaStCHEM Sch Chem, David Brewster Rd, Edinburgh EH9 3FJ, Midlothian, Scotland. EM E.Brechin@ed.ac.uk; S.J.Dalgarno@hw.ac.uk RI Dalgarno, Scott/A-7358-2010; Coletta, Marco/Q-9342-2016; Sanz, Sergio/L-5819-2016; OI Dalgarno, Scott/0000-0001-7831-012X; Coletta, Marco/0000-0003-2212-5456; McLellan, Ross/0000-0001-9700-0258 FU EPSRC [EP/I03255X/1, EP/I031421/1, EP/N004884/1]; US Department of Energy [DE-AC02-05CH11231] FX We thank the EPSRC for financial support of this work (EP/I03255X/1, EP/I031421/1 and EP/N004884/1). Mass spectrometry data was acquired at the EPSRC UK National Mass Spectrometry Facility at Swansea University. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the US Department of Energy under contract no. DE-AC02-05CH11231. NR 32 TC 1 Z9 1 U1 13 U2 24 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0947-6539 EI 1521-3765 J9 CHEM-EUR J JI Chem.-Eur. J. PD JUN 20 PY 2016 VL 22 IS 26 BP 8791 EP 8795 DI 10.1002/chem.201600762 PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA DS0FJ UT WOS:000380270500014 PM 27166930 ER PT J AU Freemire, B Tollestrup, AV Yonehara, K Chung, M Torun, Y Johnson, RP Flanagan, G Hanlet, PM Collura, MG Jana, MR Leonova, M Moretti, A Schwarz, T AF Freemire, B. Tollestrup, A. V. Yonehara, K. Chung, M. Torun, Y. Johnson, R. P. Flanagan, G. Hanlet, P. M. Collura, M. G. Jana, M. R. Leonova, M. Moretti, A. Schwarz, T. TI Pressurized rf cavities in ionizing beams SO PHYSICAL REVIEW ACCELERATORS AND BEAMS LA English DT Article ID ION-ION RECOMBINATION; ELECTRON-DRIFT VELOCITY; TOTAL CROSS-SECTIONS; DENSE GASES; OXYGEN MOLECULES; SLOW-ELECTRONS; LOW-ENERGY; DEGREES K; HYDROGEN; ATTACHMENT AB A muon collider or Higgs factory requires significant reduction of the six dimensional emittance of the beam prior to acceleration. One method to accomplish this involves building a cooling channel using high pressure gas filled radio frequency cavities. The performance of such a cavity when subjected to an intense particle beam must be investigated before this technology can be validated. To this end, a high pressure gas filled radio frequency (rf) test cell was built and placed in a 400 MeV beam line from the Fermilab linac to study the plasma evolution and its effect on the cavity. Hydrogen, deuterium, helium and nitrogen gases were studied. Additionally, sulfur hexafluoride and dry air were used as dopants to aid in the removal of plasma electrons. Measurements were made using a variety of beam intensities, gas pressures, dopant concentrations, and cavity rf electric fields, both with and without a 3 T external solenoidal magnetic field. Energy dissipation per electron-ion pair, electron-ion recombination rates, ion-ion recombination rates, and electron attachment times to SF6 and O-2 were measured. C1 [Freemire, B.; Torun, Y.; Hanlet, P. M.] IIT, Chicago, IL 60616 USA. [Tollestrup, A. V.; Yonehara, K.; Leonova, M.; Moretti, A.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Chung, M.] Uslan Natl Inst Sci & Technol, Uslan 689798, South Korea. [Johnson, R. P.; Flanagan, G.] Muons Inc, Batavia, IL 60510 USA. [Collura, M. G.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Jana, M. R.] Inst Plasma Res, Bhat 382428, Gandhinagar, India. [Schwarz, T.] Univ Michigan, Ann Arbor, MI 48109 USA. RP Freemire, B (reprint author), IIT, Chicago, IL 60616 USA. EM freeben@hawk.iit.edu FU U.S. Department of Energy [DE-AC02-07CH11359] FX The authors would like to thank the Muon Accelerator Program for making this work possible, Muons, Inc. for supplying the high pressure test cell for this experiment, the Linac crew at Fermilab for providing beam line support, and all the MTA personnel involved. Special thanks goes to Rainer Johnsen of the University of Pittsburgh, who contributed invaluable insight and with whom we had many useful discussions. Fermilab is operated by Fermi Research Alliance, LLC under Contract No. DE-AC02-07CH11359 with the U.S. Department of Energy. NR 78 TC 1 Z9 1 U1 1 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9888 J9 PHYS REV ACCEL BEAMS JI Phys. Rev. Accel. Beams PD JUN 20 PY 2016 VL 19 IS 6 AR 062004 DI 10.1103/PhysRevAccelBeams.19.062004 PG 15 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA DQ6YK UT WOS:000379352600003 ER PT J AU Ma, CH Lin, JC Liu, HJ Do, TH Zhu, YM Ha, TD Zhan, Q Juang, JY He, Q Arenholz, E Chiu, PW Chu, YH AF Ma, Chun-Hao Lin, Jheng-Cyuan Liu, Heng-Jui Thi Hien Do Zhu, Yuan-Min Thai Duy Ha Zhan, Qian Juang, Jenh-Yih He, Qing Arenholz, Elke Chiu, Po-Wen Chu, Ying-Hao TI Van der Waals epitaxy of functional MoO2 film on mica for flexible electronics SO APPLIED PHYSICS LETTERS LA English DT Article ID SINGLE-LAYER MOS2; OXIDE INTERFACES; GRAPHENE FILMS; GROWTH; TRANSPARENT; PHASE; ZNO AB Flexible electronics have a great potential to impact consumer electronics and with that our daily life. Currently, no direct growth of epitaxial functional oxides on commercially available flexible substrates is possible. In this study, in order to address this challenge, muscovite, a common layered oxide, is used as a flexible substrate that is chemically similar to typical functional oxides. We fabricated epitaxial MoO2 films on muscovite via pulsed laser deposition technique. A combination of X-ray diffraction and transmission electron microscopy confirms van der Waals epitaxy of the heterostructures. The electrical transport properties of MoO2 films are similar to those of the bulk. Flexible or free-standing MoO2 thin film can be obtained and serve as a template to integrate additional functional oxide layers. Our study demonstrates a remarkable concept to create flexible electronics based on functional oxides. Published by AIP Publishing. C1 [Ma, Chun-Hao; Chiu, Po-Wen] Natl Tsing Hua Univ, Dept Elect Engn, Hsinchu 30013, Taiwan. [Ma, Chun-Hao; Liu, Heng-Jui; Thi Hien Do; Chu, Ying-Hao] Natl Chiao Tung Univ, Dept Mat Sci & Engn, Hsinchu 30010, Taiwan. [Lin, Jheng-Cyuan; Chu, Ying-Hao] Acad Sinica, Inst Phys, Taipei 11529, Taiwan. [Zhu, Yuan-Min; Zhan, Qian] Univ Sci & Technol Beijing, Sch Mat Sci & Engn, Beijing 100083, Peoples R China. [Thai Duy Ha; Juang, Jenh-Yih; Chu, Ying-Hao] Natl Chiao Tung Univ, Dept Electrophys, Hsinchu 30010, Taiwan. [He, Qing] Univ Durham, Dept Phys, Durham DH1 3LE, England. [Arenholz, Elke] Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Chiu, Po-Wen] Acad Sinica, Inst Atom & Mol Sci, Taipei 10617, Taiwan. RP Chiu, PW (reprint author), Natl Tsing Hua Univ, Dept Elect Engn, Hsinchu 30013, Taiwan.; Chiu, PW (reprint author), Acad Sinica, Inst Atom & Mol Sci, Taipei 10617, Taiwan. EM pwchiu@ee.nthu.edu.tw; yhc@nctu.edu.tw RI He, Qing/E-3202-2010; Ying-Hao, Chu/A-4204-2008; Chiu, Po-Wen/N-7560-2015 OI Ying-Hao, Chu/0000-0002-3435-9084; FU Ministry of Science and Technology of Republic of China [MOST 103-2119-M-009-003-MY3]; Ministry of Education [MOE-ATU 101W961]; Center for Interdisciplinary Science at National Chiao Tung University; National Natural Science Foundation of China [51371031, 50971015] FX This work is supported by the Ministry of Science and Technology of Republic of China (under Contract No. MOST 103-2119-M-009-003-MY3), Ministry of Education (Grant No. MOE-ATU 101W961), and Center for Interdisciplinary Science at National Chiao Tung University. The work in University of Science and Technology Beijing is supported by the National Natural Science Foundation of China with Grant Nos. 51371031 and 50971015. NR 41 TC 2 Z9 2 U1 29 U2 54 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUN 20 PY 2016 VL 108 IS 25 AR 253104 DI 10.1063/1.4954172 PG 5 WC Physics, Applied SC Physics GA DQ2NT UT WOS:000379039900030 ER PT J AU Olson, BV Kim, JK Kadlec, EA Klem, JF Hawkins, SD Coon, WT Fortune, TR Tauke-Pedretti, A Cavaliere, MA Shaner, EA AF Olson, B. V. Kim, J. K. Kadlec, E. A. Klem, J. F. Hawkins, S. D. Coon, W. T. Fortune, T. R. Tauke-Pedretti, A. Cavaliere, M. A. Shaner, E. A. TI Optical and electrical properties of narrow-bandgap infrared W-structure superlattices incorporating AlAs/AlSb/AlAs barrier layers SO APPLIED PHYSICS LETTERS LA English DT Article AB Optical and electrical properties of nBn photodetectors using InAs/AlAs/AlSb/AlAs/InAs/InAs0.61Sb0.39W-structure superlattice (W-SL) absorbers are reported. Minority carrier lifetimes of 500 +/- 50 ns and 400 +/- 30 ns, and Auger coefficients of 2.1 x 10(-26) cm(6)/s and 1.6 x 10(-25) cm(6)/s, for samples with bandgap energies of 5.3 mu m (W-SL A) and 7.5 mu m (W-SL B) are reported at 100 K, respectively. Shockley-Read-Hall defect states are identified at 65 meV and 45 meV above the W-SL valence band edges for W-SLs A and B, respectively. Dark currents are also reported and compared with diffusion currents calculated using the carrier lifetime data, suggesting low vertical heavy hole diffusivity. Published by AIP Publishing. C1 [Olson, B. V.; Kim, J. K.; Kadlec, E. A.; Klem, J. F.; Hawkins, S. D.; Coon, W. T.; Fortune, T. R.; Tauke-Pedretti, A.; Cavaliere, M. A.; Shaner, E. A.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Olson, B. V.] Vixar Inc, 2950 Xenium Ave, Plymouth, MN 55441 USA. RP Olson, BV (reprint author), Vixar Inc, 2950 Xenium Ave, Plymouth, MN 55441 USA. EM bolson@vixarinc.com OI Olson, Benjamin/0000-0003-1421-2541 FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; U.S. Government FX Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. This work was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division and by the U.S. Government. The authors thank Dr. Ed Aifer at Naval Research Laboratories for valuable discussions on WSLs and Professor Michael Flatte at the University of Iowa for the K . p software. NR 14 TC 2 Z9 2 U1 11 U2 19 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUN 20 PY 2016 VL 108 IS 25 AR 252104 DI 10.1063/1.4954649 PG 5 WC Physics, Applied SC Physics GA DQ2NT UT WOS:000379039900017 ER PT J AU Sawada, H Lee, S Shiroto, T Nagatomo, H Arikawa, Y Nishimura, H Ueda, T Shigemori, K Sunahara, A Ohnishi, N Beg, FN Theobald, W Perez, F Patel, PK Fujioka, S AF Sawada, H. Lee, S. Shiroto, T. Nagatomo, H. Arikawa, Y. Nishimura, H. Ueda, T. Shigemori, K. Sunahara, A. Ohnishi, N. Beg, F. N. Theobald, W. Perez, F. Patel, P. K. Fujioka, S. TI Flash K alpha radiography of laser-driven solid sphere compression for fast ignition SO APPLIED PHYSICS LETTERS LA English DT Article ID HIGH-DENSITY; FUSION; HYDRODYNAMICS; PLASMAS; MATTER AB Time-resolved compression of a laser-driven solid deuterated plastic sphere with a cone was measured with flash K alpha x-ray radiography. A spherically converging shockwave launched by nanosecond GEKKO XII beams was used for compression while a flash of 4.51 keV Ti K alpha x-ray backlighter was produced by a high-intensity, picosecond laser LFEX (Laser for Fast ignition EXperiment) near peak compression for radiography. Areal densities of the compressed core were inferred from two-dimensional backlit x-ray images recorded with a narrow-band spherical crystal imager. The maximum areal density in the experiment was estimated to be 87 +/- 26 mg/cm(2). The temporal evolution of the experimental and simulated areal densities with a 2-D radiation-hydrodynamics code is in good agreement. Published by AIP Publishing. C1 [Sawada, H.] Univ Nevada, Dept Phys, Reno, NV 89557 USA. [Lee, S.; Nagatomo, H.; Arikawa, Y.; Nishimura, H.; Ueda, T.; Shigemori, K.; Fujioka, S.] Osaka Univ, Inst Laser Engn, Suita, Osaka, Japan. [Shiroto, T.; Ohnishi, N.] Tohoku Univ, Dept Aerosp Engn, Sendai, Miyagi, Japan. [Sunahara, A.] Inst Laser Technol, Nishi Ku, Osaka, Japan. [Beg, F. N.] Univ Calif San Diego, La Jolla, CA 92093 USA. [Theobald, W.] Univ Rochester, Laser Energet Lab, Rochester, NY 14623 USA. [Perez, F.] Ecole Polytech, LULI, Palaiseau, France. [Patel, P. K.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Sawada, H (reprint author), Univ Nevada, Dept Phys, Reno, NV 89557 USA. RI Patel, Pravesh/E-1400-2011; Sawada, Hiroshi/Q-8434-2016; Shigemori, Keisuke/B-3262-2013; Nishimura, Hiroaki/I-4908-2015 OI Sawada, Hiroshi/0000-0002-7972-9894; Shigemori, Keisuke/0000-0002-3978-8427; FU NIFS Collaboration Research program [NIFS13KUGK072]; UNR International Activities Grant FX This work was performed with the support and under the auspices of the NIFS Collaboration Research program (NIFS13KUGK072). The authors would like to thank the crews for the GXII and LFEX laser operation and the experimental group. H.S. acknowledged the support by the UNR International Activities Grant. NR 33 TC 0 Z9 0 U1 5 U2 6 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUN 20 PY 2016 VL 108 IS 25 AR 254101 DI 10.1063/1.4954383 PG 4 WC Physics, Applied SC Physics GA DQ2NT UT WOS:000379039900046 ER PT J AU Yang, SM Mazet, L Okatan, MB Jesse, S Niu, G Schroeder, T Schamm-Chardon, S Dubourdieu, C Baddorf, AP Kalinin, SV AF Yang, Sang Mo Mazet, Lucie Okatan, M. Baris Jesse, Stephen Niu, Gang Schroeder, Thomas Schamm-Chardon, Sylvie Dubourdieu, Catherine Baddorf, Arthur P. Kalinin, Sergei V. TI Decoupling indirect topographic cross-talk in band excitation piezoresponse force microscopy imaging and spectroscopy SO APPLIED PHYSICS LETTERS LA English DT Article ID RESOLUTION AB All scanning probe microscopies are subjected to topographic cross-talk, meaning the topography-related contrast in functional images. Here, we investigate the signatures of indirect topographic cross-talk in piezoresponse force microscopy (PFM) imaging and spectroscopy and its decoupling using band excitation (BE) method in ferroelectric BaTiO3 deposited on the Si substrates with free standing nanopillars of diameter 50 nm. Comparison between the single-frequency PFM and BE-PFM results shows that the measured signal can be significantly distorted by topography-induced shifts in the contact resonance frequency and cantilever transfer function. However, with proper correction, such shifts do not affect PFM imaging and hysteresis loop measurements. This suggests the necessity of an advanced approach, such as BE-PFM, for detection of intrinsic sample piezoresponse on the topographically non-uniform surfaces. Published by AIP Publishing. C1 [Yang, Sang Mo; Okatan, M. Baris; Jesse, Stephen; Baddorf, Arthur P.; Kalinin, Sergei V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Mazet, Lucie; Dubourdieu, Catherine] Univ Lyon, Ecole Cent Lyon, Inst Nanotechnol Lyon, CNRS,UMR 5270, F-69134 Ecully, France. [Niu, Gang; Schroeder, Thomas] IHP Innovat High Performance Microelect, Technol Pk 25, D-15236 Frankfurt, Germany. [Schamm-Chardon, Sylvie] Univ Toulouse, CNRS, CEMES, 29 Rue Jeanne Marvig, F-31055 Toulouse, France. [Niu, Gang] Xi An Jiao Tong Univ, Elect Mat Res Lab, Key Lab, Minist Educ, Xian 710049, Peoples R China. [Niu, Gang] Xi An Jiao Tong Univ, Int Ctr Dielect Res, Xian 710049, Peoples R China. [Dubourdieu, Catherine] Helmholtz Zentrum Berlin Mat & Energie, IFOX, Hahn Meitner Pl 1, D-14109 Berlin, Germany. RP Yang, SM; Kalinin, SV (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM yangs@ornl.gov; sergei2@ornl.gov RI Okatan, M. Baris/E-1913-2016; Yang, Sang Mo/Q-2455-2015; OI Okatan, M. Baris/0000-0002-9421-7846; Yang, Sang Mo/0000-0003-1809-2938; Schamm-Chardon, Sylvie/0000-0001-5534-8475 FU LABEX iMUST of Universite de Lyon, within the program "Investissements d'Avenir" [ANR-10-LABX-0064, ANR-11-IDEX-0007]; project INTENSE [ANR-14-CE26-0010] FX Data acquisition, analysis, and methods (S.M.Y., M.B.O., S.J., A.P.B., and S.V.K.) were supported by and conducted at the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. Materials synthesis work (L.M. and C.D.) was supported by the LABEX iMUST (ANR-10-LABX-0064) of Universite de Lyon, within the program "Investissements d'Avenir" (ANR-11-IDEX-0007) operated by the French National Research Agency (ANR) and, together with the TEM work as well (S.S.-C.), by the Grant No. ANR-14-CE26-0010 (project INTENSE). Robin Cours from CEMES is acknowledged for his strong support on the TEM sample preparation. NR 20 TC 0 Z9 0 U1 6 U2 16 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUN 20 PY 2016 VL 108 IS 25 AR 252902 DI 10.1063/1.4954276 PG 5 WC Physics, Applied SC Physics GA DQ2NT UT WOS:000379039900025 ER PT J AU Corrochano, LM Kuo, A Marcet-Houben, M Polaino, S Salamov, A Villalobos-Escobedo, JM Grimwood, J Alvarez, MI Avalos, J Bauer, D Benito, EP Benoit, I Burger, G Camino, LP Canovas, D Cerda-Olmedo, E Cheng, JF Dominguez, A Elias, M Eslava, AP Glaser, F Gutierrez, G Heitman, J Henrissat, B Iturriaga, EA Lang, BF Lavin, JL Lee, SC Li, WJ Lindquist, E Lopez-Garcia, S Luque, EM Marcos, AT Martin, J McCluskey, K Medina, HR Miralles-Duran, A Miyazaki, A Munoz-Torres, E Oguiza, JA Ohm, RA Olmedo, M Orejas, M Ortiz-Castellanos, L Pisabarro, AG Rodriguez-Romero, J Ruiz-Herrera, J Ruiz-Vazquez, R Sanz, C Schackwitz, W Shahriari, M Shelest, E Silva-Franco, F Soanes, D Syed, K Tagua, VG Talbot, NJ Thon, MR Tice, H de Vries, RP Wiebenga, A Yadav, JS Braun, EL Baker, SE Garre, V Schmutz, J Horwitz, BA Torres-Martinez, S Idnurm, A Herrera-Estrella, A Gabaldon, T Grigoriev, IV AF Corrochano, Luis M. Kuo, Alan Marcet-Houben, Marina Polaino, Silvia Salamov, Asaf Villalobos-Escobedo, Jose M. Grimwood, Jane Isabel Alvarez, M. Avalos, Javier Bauer, Diane Benito, Ernesto P. Benoit, Isabelle Burger, Gertraud Camino, Lola P. Canovas, David Cerda-Olmedo, Enrique Cheng, Jan-Fang Dominguez, Angel Elias, Marek Eslava, Arturo P. Glaser, Fabian Gutierrez, Gabriel Heitman, Joseph Henrissat, Bernard Iturriaga, Enrique A. Lang, B. Franz Lavin, Jose L. Lee, Soo Chan Li, Wenjun Lindquist, Erika Lopez-Garcia, Sergio Luque, Eva M. Marcos, Ana T. Martin, Joel McCluskey, Kevin Medina, Humberto R. Miralles-Duran, Alejandro Miyazaki, Atsushi Munoz-Torres, Elisa Oguiza, Jose A. Ohm, Robin A. Olmedo, Maria Orejas, Margarita Ortiz-Castellanos, Lucila Pisabarro, Antonio G. Rodriguez-Romero, Julio Ruiz-Herrera, Jose Ruiz-Vazquez, Rosa Sanz, Catalina Schackwitz, Wendy Shahriari, Mahdi Shelest, Ekaterina Silva-Franco, Fatima Soanes, Darren Syed, Khajamohiddin Tagua, Victor G. Talbot, Nicholas J. Thon, Michael R. Tice, Hope de Vries, Ronald P. Wiebenga, Ad Yadav, Jagjit S. Braun, Edward L. Baker, Scott E. Garre, Victoriano Schmutz, Jeremy Horwitz, Benjamin A. Torres-Martinez, Santiago Idnurm, Alexander Herrera-Estrella, Alfredo Gabaldon, Toni Grigoriev, Igor V. TI Expansion of Signal Transduction Pathways in Fungi by Extensive Genome Duplication SO CURRENT BIOLOGY LA English DT Article ID G-PROTEIN; SACCHAROMYCES-CEREVISIAE; MUCOR-CIRCINELLOIDES; LIGHT RESPONSES; PHYCOMYCES; PHOTORECEPTOR; PHOTOTROPISM; GENES; MUTANTS; MADA AB Plants and fungi use light and other signals to regulate development, growth, and metabolism. The fruiting bodies of the fungus Phycomyces blakesleeanus are single cells that react to environmental cues, including light, but the mechanisms are largely unknown [1]. The related fungus Mucor circinelloides is an opportunistic human pathogen that changes its mode of growth upon receipt of signals from the environment to facilitate pathogenesis [2]. Understanding how these organisms respond to environmental cues should provide insights into the mechanisms of sensory perception and signal transduction by a single eukaryotic cell, and their role in pathogenesis. We sequenced the genomes of P. blakesleeanus and M. circinelloides and show that they have been shaped by an extensive genome duplication or, most likely, a whole-genome duplication (WGD), which is rarely observed in fungi [3-6]. We show that the genome duplication has expanded gene families, including those involved in signal transduction, and that duplicated genes have specialized, as evidenced by differences in their regulation by light. The transcriptional response to light varies with the developmental stage and is still observed in a photoreceptor mutant of P. blakesleeanus. A phototropic mutant of P. blakesleeanus with a heterozygous mutation in the photoreceptor gene madA demonstrates that photosensor dosage is important for the magnitude of signal transduction. We conclude that the genome duplication provided the means to improve signal transduction for enhanced perception of environmental signals. Our results will help to understand the role of genome dynamics in the evolution of sensory perception in eukaryotes. C1 [Corrochano, Luis M.; Avalos, Javier; Camino, Lola P.; Canovas, David; Cerda-Olmedo, Enrique; Gutierrez, Gabriel; Luque, Eva M.; Marcos, Ana T.; Medina, Humberto R.; Miralles-Duran, Alejandro; Olmedo, Maria; Rodriguez-Romero, Julio; Tagua, Victor G.] Univ Seville, Dept Genet, Ave Reina Mercedes S-N, E-41012 Seville, Spain. [Kuo, Alan; Salamov, Asaf; Grimwood, Jane; Bauer, Diane; Cheng, Jan-Fang; Lindquist, Erika; Martin, Joel; Ohm, Robin A.; Schackwitz, Wendy; Tice, Hope; Schmutz, Jeremy; Grigoriev, Igor V.] US DOE, Joint Genome Inst, 2800 Mitchell Dr, Walnut Creek, CA 94598 USA. [Marcet-Houben, Marina; Gabaldon, Toni] Ctr Genom Regulat CRG, Doctor Aiguader 88, Barcelona 08003, Spain. [Marcet-Houben, Marina; Gabaldon, Toni] Univ Pompeu Fabra UPF, Doctor Aiguader 88, Barcelona 08003, Spain. [Polaino, Silvia; Idnurm, Alexander] Univ Missouri, Sch Biol Sci, 5007 Rockhill Rd, Kansas City, MO 64110 USA. [Villalobos-Escobedo, Jose M.; Herrera-Estrella, Alfredo] Ctr Invest & Estudios Avanzados, Lab Nacl Genom Biodiversidad LANGEBIO, Kilometro 9-6 Libramiento Norte, Guanajuato 36821, Mexico. [Grimwood, Jane; Schmutz, Jeremy] HudsonAlpha Inst Biotechnol, 601 Genome Way Northwest, Huntsville, AL 35806 USA. [Isabel Alvarez, M.; Benito, Ernesto P.; Dominguez, Angel; Eslava, Arturo P.; Iturriaga, Enrique A.; Sanz, Catalina; Shahriari, Mahdi; Thon, Michael R.] Univ Salamanca, Dept Microbiol & Genet, Plaza Doctores Reina S-N, Salamanca 37007, Spain. [Benito, Ernesto P.; Thon, Michael R.] Univ Salamanca, Inst Hispanoluso Invest Agr CIALE, Rio Duero 12, Salamanca 37185, Spain. [Benoit, Isabelle; de Vries, Ronald P.; Wiebenga, Ad] Univ Utrecht, CBS KNAW Fungal Biodivers Ctr, Uppsalalaan 8, NL-3584 CT Utrecht, Netherlands. [Benoit, Isabelle; de Vries, Ronald P.; Wiebenga, Ad] Univ Utrecht, Fungal Mol Physiol, Uppsalalaan 8, NL-3584 CT Utrecht, Netherlands. [Burger, Gertraud; Lang, B. Franz] Univ Montreal, Pavillon Roger Gaudry,Biochimie,CP 6128, Montreal, PQ H3C 3J7, Canada. [Elias, Marek] Univ Ostrava, Fac Sci, Dept Biol & Ecol, Chittussiho 10, Ostrava 71000, Czech Republic. [Glaser, Fabian] Technion Israel Inst Technol, Lokey Interdisciplinary Ctr Life Sci & Engn, IL-3200003 Haifa, Israel. [Heitman, Joseph; Lee, Soo Chan; Li, Wenjun] Duke Univ, Med Ctr, Dept Mol Genet & Microbiol, Res Dr, Durham, NC 27710 USA. [Henrissat, Bernard] Univ Aix Marseille, UMR7257, CNRS, 163 Ave Luminy, F-13288 Marseille, France. [Henrissat, Bernard] King Abdulaziz Univ, Dept Biol Sci, POB 80203, Jeddah 21589, Saudi Arabia. [Lavin, Jose L.] CIC BioGUNE, Genome Anal Platform, Bizkaia Technol Pk, Derio 48160, Bizkaia, Spain. [Lopez-Garcia, Sergio; Ruiz-Vazquez, Rosa; Silva-Franco, Fatima; Garre, Victoriano; Torres-Martinez, Santiago] Univ Murcia, Dept Genet & Microbiol, E-30071 Murcia, Spain. [McCluskey, Kevin] Kansas State Univ, Dept Plant Pathol, 4024 Throckmorton Plant Sci Ctr, Manhattan, KS 66506 USA. [Miyazaki, Atsushi] Ishinomaki Senshu Univ, Dept Biol Sci, Fac Sci & Engn, Ishinomaki, Miyagi 9868580, Japan. [Munoz-Torres, Elisa] Univ Salamanca, Fac Med, Dept Biol Celular & Patol, Ave Campus Miguel de Unamuno, Salamanca 37007, Spain. [Oguiza, Jose A.; Pisabarro, Antonio G.] Univ Publ Navarra, Dept Agr Prod, Pamplona 31006, Spain. [Orejas, Margarita] Consejo Super Invest Cient IATA CSIC, Inst Agroquim & Tecnol Alimentos, Ave Catedrat Agustin Escardino 7, Valencia 46980, Spain. [Ortiz-Castellanos, Lucila; Ruiz-Herrera, Jose] Inst Politecn Nacl, Ctr Invest & Estudios Avanzados, Unidad Irapuato, Dept Ingn Genet, Kilometro 9-6 Libramiento Norte, Guanajuato 36821, Mexico. [Shelest, Ekaterina] Hans Knoell Inst, Leibniz Inst Nat Prod Res & Infect Biol, Beutenbergstr 11a, D-07745 Jena, Germany. [Soanes, Darren; Talbot, Nicholas J.] Univ Exeter, Coll Life & Environm Sci, Biosci, Stocker Rd, Exeter EX4 4QD, Devon, England. [Syed, Khajamohiddin; Yadav, Jagjit S.] Univ Cincinnati, Coll Med, Dept Environm Hlth, 160 Panzeca Way, Cincinnati, OH 45267 USA. [Braun, Edward L.] Univ Florida, Dept Biol, POB 118525, Gainesville, FL 32611 USA. [Baker, Scott E.] Pacific NW Natl Lab, 902 Battelle Blvd, Richland, WA 99352 USA. [Horwitz, Benjamin A.] Technion Israel Inst Technol, Dept Biol, IL-32000 Haifa, Israel. [Idnurm, Alexander] Univ Melbourne, Sch BioSci, Melbourne, Vic 3010, Australia. [Gabaldon, Toni] ICREA, Barcelona 08010, Spain. RP Corrochano, LM (reprint author), Univ Seville, Dept Genet, Ave Reina Mercedes S-N, E-41012 Seville, Spain. EM corrochano@us.es RI Olmedo, Maria/E-1824-2012; Benito, Ernesto/B-5437-2017; Corrochano, Luis/F-5720-2010; Ohm, Robin/I-6689-2016; Elias, Marek/D-6851-2014; Idnurm, Alexander/K-8558-2013; de Vries, Ronald/F-8125-2011; Camino, Lola/C-2150-2017; Herrera-Estrella, Alfredo/F-3185-2011; Thon, Michael/M-9463-2014; Canovas, David/L-7628-2014; Schmutz, Jeremy/N-3173-2013; Avalos, Javier/B-4218-2011; Fac Sci, KAU, Biol Sci Dept/L-4228-2013; OI Olmedo, Maria/0000-0002-5701-2665; Benito, Ernesto/0000-0002-9873-0970; Corrochano, Luis/0000-0002-6282-6567; Elias, Marek/0000-0003-0066-6542; Idnurm, Alexander/0000-0001-5995-7040; de Vries, Ronald/0000-0002-4363-1123; Herrera-Estrella, Alfredo/0000-0002-4589-6870; Thon, Michael/0000-0002-7225-7003; Canovas, David/0000-0002-7293-7332; Schmutz, Jeremy/0000-0001-8062-9172; Avalos, Javier/0000-0001-5484-2893; Braun, Edward/0000-0003-1643-5212; Silva-Franco, Fatima/0000-0002-2900-027X; Lavin, Jose Luis/0000-0003-0914-3211 FU NIAID NIH HHS [R01 AI050113] NR 33 TC 12 Z9 12 U1 11 U2 20 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0960-9822 EI 1879-0445 J9 CURR BIOL JI Curr. Biol. PD JUN 20 PY 2016 VL 26 IS 12 BP 1577 EP 1584 DI 10.1016/j.cub.2016.04.038 PG 8 WC Biochemistry & Molecular Biology; Cell Biology SC Biochemistry & Molecular Biology; Cell Biology GA DP7EK UT WOS:000378661800022 PM 27238284 ER PT J AU Kearney, SP Guildenbecher, DR AF Kearney, Sean P. Guildenbecher, Daniel R. TI Temperature measurements in metalized propellant combustion using hybrid fs/ps coherent anti-Stokes Raman scattering SO APPLIED OPTICS LA English DT Article ID GAS-PHASE THERMOMETRY; IN-LINE HOLOGRAPHY; AMMONIUM-PERCHLORATE; ELEVATED PRESSURE; CARS MEASUREMENTS; SOOTING FLAMES; SPECTROSCOPY; INTERFERENCE; PROBE; DECOMPOSITION AB We apply ultrafast pure-rotational coherent anti-Stokes Raman scattering (CARS) for temperature and relative oxygen concentration measurements in the plume emanating from a burning, aluminized ammonium-perchlorate propellant strand. Combustion of these metal-based propellants is a particularly hostile environment for laser-based diagnostics, with intense background luminosity and scattering from hot metal particles as large as several hundred micrometers in diameter. CARS spectra that were previously obtained using nanosecond pulsed lasers in an aluminum-particle-seeded flame are examined and are determined to be severely impacted by nonresonant background, presumably as a result of the plasma formed by particulate-enhanced laser-induced breakdown. Introduction of femtosecond/picosecond (fs/ps) laser pulses improves CARS detection by providing time-gated elimination of strong nonresonant background interference. Single-laser-shot fs/ps CARS spectra were acquired from the burning propellant plume, with picosecond probe-pulse delays of 0 and 16 ps from the femtosecond pump and Stokes pulses. At zero delay, nonresonant background overwhelms the Raman-resonant spectroscopic features. Time-delayed probing results in the acquisition of background-free spectra that were successfully fit for temperature and relative oxygen content. Temperature probability densities and temperature/oxygen correlations were constructed from ensembles of several thousand single-laser-shot measurements with the CARS measurement volume positioned within 3 mm or less of the burning propellant surface. The results show that ultrafast CARS is a potentially enabling technology for probing harsh, particle-laden flame environments. C1 [Kearney, Sean P.; Guildenbecher, Daniel R.] Sandia Natl Labs, Engn Sci Ctr, POB 5800, Albuquerque, NM 87185 USA. RP Kearney, SP (reprint author), Sandia Natl Labs, Engn Sci Ctr, POB 5800, Albuquerque, NM 87185 USA. EM spkearn@sandia.gov FU Sandia National Laboratories [DE-AC04-94AL85000] FX Sandia National Laboratories (DE-AC04-94AL85000). NR 49 TC 0 Z9 0 U1 9 U2 12 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1559-128X EI 2155-3165 J9 APPL OPTICS JI Appl. Optics PD JUN 20 PY 2016 VL 55 IS 18 BP 4958 EP 4966 DI 10.1364/AO.55.004958 PG 9 WC Optics SC Optics GA DO8ZZ UT WOS:000378075400027 PM 27409125 ER PT J AU Aartsen, MG Abraham, K Ackermann, M Adams, J Aguilar, JA Ahlers, M Ahrens, M Altmann, D Andeen, K Anderson, T Ansseau, I Anton, G Archinger, M Arguelles, C Arlen, TC Auffenberg, J Bai, X Barwick, SW Baum, V Bay, R Beatty, JJ Tjus, JB Becker, KH BenZvi, S Berghaus, P Berley, D Bernardini, E Bernhard, A Besson, DZ Binder, G Bindig, D Bissok, M Blaufuss, E Blot, S Boersma, DJ Bohm, C Borner, M Bos, F Bose, D Boser, S Botner, O Braun, J Brayeur, L Bretz, HP Burgman, A Buzinsky, N Casey, J Casier, M Cheung, E Chirkin, D Christov, A Clark, K Classen, L Coenders, S Collin, GH Conrad, JM Cowen, DF Silva, AHC Daughhetee, J Davis, JC Day, M de Andre, JPAM De Clercq, C Rosendo, ED Dembinski, H De Ridder, S Desiati, P de Vries, KD de Wasseige, G de With, M DeYoung, T Diaz-Velez, JC di Lorenzo, V Dujmovic, H Dumm, JP Dunkman, M Eberhardt, B Ehrhardt, T Eichmann, B Euler, S Evenson, PA Fahey, S Fazely, AR Feintzeig, J Felde, J Filimonov, K Finley, C Flis, S Fosig, CC Fuchs, T Gaisser, TK Gaior, R Gallagher, J Gerhardt, L Ghorbani, K Gladstone, L Glagla, M Glusenkamp, T Goldschmidt, A Golup, G Gonzalez, JG Gora, D Grant, D Griffith, Z Ha, C Haack, C Ismail, AH Hallgren, A Halzen, F Hansen, E Hansmann, B Hansmann, T Hanson, K Hebecker, D Heereman, D Helbing, K Hellauer, R Hickford, S Hignight, J Hill, GC Hoffman, KD Hoffmann, R Holzapfel, K Homeier, A Hoshina, K Huang, F Huber, M Huelsnitz, W Hultqvist, K In, S Ishihara, A Jacobi, E Japaridze, GS Jeong, M Jero, K Jones, BJP Jurkovic, M Kappes, A Karg, T Karle, A Katz, U Kauer, M Keivani, A Kelley, JL Kemp, J Kheirandish, A Kim, M Kintscher, T Kiryluk, J Klein, SR Kohnen, G Koirala, R Kolanoski, H Konietz, R Kopke, L Kopper, C Kopper, S Koskinen, DJ Kowalski, M Krings, K Kroll, M Kruckl, G Kruger, C Kunnen, J Kunwar, S Kurahashi, N Kuwabara, T Labare, M Lanfranchi, JL Larson, MJ Lennarz, D Lesiak-Bzdak, M Leuermann, M Leuner, J Lu, L Lunemann, J Madsen, J Maggi, G Mahn, KBM Mancina, S Mandelartz, M Maruyama, R Mase, K Matis, HS Maunu, R McNally, F Meagher, K Medici, M Meier, M Meli, A Menne, T Merino, G Meures, T Miarecki, S Middell, E Mohrmann, L Montaruli, T Nahnhauer, R Naumann, U Neer, G Niederhausen, H Nowicki, SC Nygren, DR Pollmann, AO Olivas, A Omairat, A O'Murchadha, A Palczewski, T Pandya, H Pankova, DV Penek, O Pepper, JA de los Heros, CP Pfendner, C Pieloth, D Pinat, E Posselt, J Price, PB Przybylski, GT Quinnan, M Raab, C Radel, L Rameez, M Rawlins, K Reimann, R Relich, M Resconi, E Rhode, W Richman, M Riedel, B Robertson, S Rongen, M Rott, C Ruhe, T Ryckbosch, D Sabbatini, L Sandrock, A Sandroos, J Sarkar, S Satalecka, K Schimp, M Schlunder, P Schmidt, T Schoenen, S Schoneberg, S Schonwald, A Schumacher, L Seckel, D Seunarine, S Soldin, D Song, M Spiczak, GM Spiering, C Stahlberg, M Stamatikos, M Stanev, T Stasik, A Steuer, A Stezelberger, T Stokstad, RG Stossl, A Strom, R Strotjohann, NL Sullivan, GW Sutherland, M Taavola, H Taboada, I Tatar, J Ter-Antonyan, S Terliuk, A Tesic, G Tilav, S Toale, PA Tobin, MN Toscano, S Tosi, D Tselengidou, M Turcati, A Unger, E Usner, M Vallecorsa, S Vandenbroucke, J van Eijndhoven, N Vanheule, S van Rossem, M van Santen, J Veenkamp, J Vehring, M Voge, M Vraeghe, M Walck, C Wallace, A Wallraff, M Wandkowsky, N Weaver, C Wendt, C Westerhoff, S Whelan, BJ Whitehorn, N Wickmann, S Wiebe, K Wiebusch, CH Wille, L Williams, DR Wills, L Wissing, H Wolf, M Wood, TR Woschnagg, K Xu, DL Xu, XW Xu, Y Yanez, JP Yodh, G Yoshida, S Zoll, M AF Aartsen, M. G. Abraham, K. Ackermann, M. Adams, J. Aguilar, J. A. Ahlers, M. Ahrens, M. Altmann, D. Andeen, K. Anderson, T. Ansseau, I. Anton, G. Archinger, M. Arguelles, C. Arlen, T. C. Auffenberg, J. Bai, X. Barwick, S. W. Baum, V. Bay, R. Beatty, J. J. Tjus, J. Becker Becker, K. -H. BenZvi, S. Berghaus, P. Berley, D. Bernardini, E. Bernhard, A. Besson, D. Z. Binder, G. Bindig, D. Bissok, M. Blaufuss, E. Blot, S. Boersma, D. J. Bohm, C. Boerner, M. Bos, F. Bose, D. Boeser, S. Botner, O. Braun, J. Brayeur, L. Bretz, H. -P. Burgman, A. Buzinsky, N. Casey, J. Casier, M. Cheung, E. Chirkin, D. Christov, A. Clark, K. Classen, L. Coenders, S. Collin, G. H. Conrad, J. M. Cowen, D. F. Silva, A. H. Cruz Daughhetee, J. Davis, J. C. Day, M. de Andre, J. P. A. M. De Clercq, C. del Pino Rosendo, E. Dembinski, H. De Ridder, S. Desiati, P. de Vries, K. D. de Wasseige, G. de With, M. DeYoung, T. Diaz-Velez, J. C. di Lorenzo, V. Dujmovic, H. Dumm, J. P. Dunkman, M. Eberhardt, B. Ehrhardt, T. Eichmann, B. Euler, S. Evenson, P. A. Fahey, S. Fazely, A. R. Feintzeig, J. Felde, J. Filimonov, K. Finley, C. Flis, S. Foesig, C. -C. Fuchs, T. Gaisser, T. K. Gaior, R. Gallagher, J. Gerhardt, L. Ghorbani, K. Gladstone, L. Glagla, M. Gluesenkamp, T. Goldschmidt, A. Golup, G. Gonzalez, J. G. Gora, D. Grant, D. Griffith, Z. Ha, C. Haack, C. Ismail, A. Haj Hallgren, A. Halzen, F. Hansen, E. Hansmann, B. Hansmann, T. Hanson, K. Hebecker, D. Heereman, D. Helbing, K. Hellauer, R. Hickford, S. Hignight, J. Hill, G. C. Hoffman, K. D. Hoffmann, R. Holzapfel, K. Homeier, A. Hoshina, K. Huang, F. Huber, M. Huelsnitz, W. Hultqvist, K. In, S. Ishihara, A. Jacobi, E. Japaridze, G. S. Jeong, M. Jero, K. Jones, B. J. P. Jurkovic, M. Kappes, A. Karg, T. Karle, A. Katz, U. Kauer, M. Keivani, A. Kelley, J. L. Kemp, J. Kheirandish, A. Kim, M. Kintscher, T. Kiryluk, J. Klein, S. R. Kohnen, G. Koirala, R. Kolanoski, H. Konietz, R. Koepke, L. Kopper, C. Kopper, S. Koskinen, D. J. Kowalski, M. Krings, K. Kroll, M. Kruckl, G. Krueger, C. Kunnen, J. Kunwar, S. Kurahashi, N. Kuwabara, T. Labare, M. Lanfranchi, J. L. Larson, M. J. Lennarz, D. Lesiak-Bzdak, M. Leuermann, M. Leuner, J. Lu, L. Luenemann, J. Madsen, J. Maggi, G. Mahn, K. B. M. Mancina, S. Mandelartz, M. Maruyama, R. Mase, K. Matis, H. S. Maunu, R. McNally, F. Meagher, K. Medici, M. Meier, M. Meli, A. Menne, T. Merino, G. Meures, T. Miarecki, S. Middell, E. Mohrmann, L. Montaruli, T. Nahnhauer, R. Naumann, U. Neer, G. Niederhausen, H. Nowicki, S. C. Nygren, D. R. Pollmann, A. Obertacke Olivas, A. Omairat, A. O'Murchadha, A. Palczewski, T. Pandya, H. Pankova, D. V. Penek, O. Pepper, J. A. de los Heros, C. Perez Pfendner, C. Pieloth, D. Pinat, E. Posselt, J. Price, P. B. Przybylski, G. T. Quinnan, M. Raab, C. Raedel, L. Rameez, M. Rawlins, K. Reimann, R. Relich, M. Resconi, E. Rhode, W. Richman, M. Riedel, B. Robertson, S. Rongen, M. Rott, C. Ruhe, T. Ryckbosch, D. Sabbatini, L. Sandrock, A. Sandroos, J. Sarkar, S. Satalecka, K. Schimp, M. Schlunder, P. Schmidt, T. Schoenen, S. Schoeneberg, S. Schoenwald, A. Schumacher, L. Seckel, D. Seunarine, S. Soldin, D. Song, M. Spiczak, G. M. Spiering, C. Stahlberg, M. Stamatikos, M. Stanev, T. Stasik, A. Steuer, A. Stezelberger, T. Stokstad, R. G. Stossl, A. Stroem, R. Strotjohann, N. L. Sullivan, G. W. Sutherland, M. Taavola, H. Taboada, I. Tatar, J. Ter-Antonyan, S. Terliuk, A. Tesic, G. Tilav, S. Toale, P. A. Tobin, M. N. Toscano, S. Tosi, D. Tselengidou, M. Turcati, A. Unger, E. Usner, M. Vallecorsa, S. Vandenbroucke, J. van Eijndhoven, N. Vanheule, S. van Rossem, M. van Santen, J. Veenkamp, J. Vehring, M. Voge, M. Vraeghe, M. Walck, C. Wallace, A. Wallraff, M. Wandkowsky, N. Weaver, Ch Wendt, C. Westerhoff, S. Whelan, B. J. Whitehorn, N. Wickmann, S. Wiebe, K. Wiebusch, C. H. Wille, L. Williams, D. R. Wills, L. Wissing, H. Wolf, M. Wood, T. R. Woschnagg, K. Xu, D. L. Xu, X. W. Xu, Y. Yanez, J. P. Yodh, G. Yoshida, S. Zoll, M. CA IceCube Collaboration TI LOWERING ICECUBE'S ENERGY THRESHOLD FOR POINT SOURCE SEARCHES IN THE SOUTHERN SKY SO ASTROPHYSICAL JOURNAL LETTERS LA English DT Article DE astroparticle physics; neutrinos ID COSMIC-RAYS; GAMMA-RAY; NEUTRINO TELESCOPE; ASTROPHYSICS AB Observation of a point source of astrophysical neutrinos would be a "smoking gun" signature of a cosmic-ray accelerator. While IceCube has recently discovered a diffuse flux of astrophysical neutrinos, no localized point source has been observed. Previous IceCube searches for point sources in the southern sky were restricted by either an energy threshold above a few hundred TeV or poor neutrino angular resolution. Here we present a search for southern sky point sources with greatly improved sensitivities to neutrinos with energies below 100 TeV. By selecting charged-current nu(mu) interacting inside the detector, we reduce the atmospheric background while retaining efficiency for astrophysical neutrino-induced events reconstructed with sub-degree angular resolution. The new event sample covers three years of detector data and leads to a factor of 10 improvement in sensitivity to point sources emitting below 100 TeV in the southern sky. No statistically significant evidence of point sources was found, and upper limits are set on neutrino emission from individual sources. A posteriori analysis of the highest-energy (similar to 100 TeV) starting event in the sample found that this event alone represents a 2.8 sigma deviation from the hypothesis that the data consists only of atmospheric background. C1 [Aartsen, M. G.; Hill, G. C.; Robertson, S.; Wallace, A.; Whelan, B. J.] Univ Adelaide, Dept Phys, Adelaide, SA 5005, Australia. 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C.; Fahey, S.; Feintzeig, J.; Ghorbani, K.; Gladstone, L.; Griffith, Z.; Halzen, F.; Hanson, K.; Hoshina, K.; Jero, K.; Karle, A.; Kauer, M.; Kelley, J. L.; Kheirandish, A.; Krueger, C.; Mancina, S.; McNally, F.; Merino, G.; Sabbatini, L.; Tobin, M. N.; Tosi, D.; Vandenbroucke, J.; van Rossem, M.; Wandkowsky, N.; Wendt, C.; Westerhoff, S.; Wille, L.; Xu, D. L.] Univ Wisconsin, Dept Phys, 1150 Univ Ave, Madison, WI 53706 USA. [Braun, J.; Chirkin, D.; Day, M.; Desiati, P.; Diaz-Velez, J. C.; Fahey, S.; Feintzeig, J.; Ghorbani, K.; Gladstone, L.; Griffith, Z.; Halzen, F.; Hanson, K.; Hoshina, K.; Jero, K.; Karle, A.; Kauer, M.; Kelley, J. L.; Kheirandish, A.; Krueger, C.; Mancina, S.; McNally, F.; Merino, G.; Sabbatini, L.; Tobin, M. N.; Tosi, D.; Vandenbroucke, J.; van Rossem, M.; Wandkowsky, N.; Wendt, C.; Westerhoff, S.; Wille, L.; Xu, D. L.] Univ Wisconsin, Wisconsin IceCube Particle Astrophys Ctr, Madison, WI USA. [Ahrens, M.; Bohm, C.; Dumm, J. 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[Binder, G.; Gerhardt, L.; Goldschmidt, A.; Ha, C.; Klein, S. R.; Matis, H. S.; Miarecki, S.; Nygren, D. R.; Przybylski, G. T.; Stezelberger, T.; Stokstad, R. G.; Tatar, J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Boersma, D. J.; Botner, O.; Burgman, A.; Euler, S.; Hallgren, A.; de los Heros, C. Perez; Stroem, R.; Taavola, H.; Unger, E.] Uppsala Univ, Dept Phys & Astron, Box 516, S-75120 Uppsala, Sweden. [Bose, D.; Dujmovic, H.; In, S.; Jeong, M.; Kim, M.; Rott, C.] TU Dortmund Univ, Dept Phys, D-44221 Dortmund, Germany. [Brayeur, L.; Casier, M.; De Clercq, C.; de Vries, K. D.; de Wasseige, G.; Golup, G.; Kunnen, J.; Luenemann, J.; Maggi, G.; Toscano, S.; van Eijndhoven, N.] Vrije Univ Brussel, Dienst ELEM, B-1050 Brussels, Belgium. [Buzinsky, N.; Grant, D.; Kopper, C.; Nowicki, S. C.; Riedel, B.; Weaver, Ch; Wood, T. R.] Univ Alberta, Dept Phys, Edmonton, AB T6G 2E1, Canada. [Casey, J.; Daughhetee, J.; Taboada, I.] Georgia Inst Technol, Sch Phys, Atlanta, GA 30332 USA. [Casey, J.; Daughhetee, J.; Taboada, I.] Georgia Inst Technol, Ctr Relativist Astrophys, Atlanta, GA 30332 USA. [Christov, A.; Montaruli, T.; Rameez, M.; Vallecorsa, S.] Univ Geneva, Dept Phys Nucl & Corpusculaire, CH-1211 Geneva, Switzerland. [Clark, K.] Univ Toronto, Dept Phys, 60 St George St, Toronto, ON M5S 1A7, Canada. [Cowen, D. F.] Penn State Univ, Dept Astron & Astrophys, 525 Davey Lab, University Pk, PA 16802 USA. [de Andre, J. P. A. M.; DeYoung, T.; Hignight, J.; Lennarz, D.; Mahn, K. B. M.; Neer, G.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Dembinski, H.; Evenson, P. A.; Gaisser, T. K.; Gonzalez, J. G.; Koirala, R.; Pandya, H.; Seckel, D.; Stanev, T.; Tilav, S.] Univ Delaware, Bartol Res Inst, Newark, DE 19716 USA. [Dembinski, H.; Evenson, P. A.; Gaisser, T. K.; Gonzalez, J. G.; Koirala, R.; Pandya, H.; Seckel, D.; Stanev, T.; Tilav, S.] Univ Delaware, Dept Phys & Astron, Newark, DE 19716 USA. [De Ridder, S.; Ismail, A. Haj; Labare, M.; Meli, A.; Ryckbosch, D.; Vanheule, S.; Vraeghe, M.] Univ Ghent, Dept Phys & Astron, B-9000 Ghent, Belgium. [de With, M.; Hebecker, D.; Kolanoski, H.; Kowalski, M.] Humboldt Univ, Inst Phys, D-12489 Berlin, Germany. [Gaior, R.; Ishihara, A.; Kuwabara, T.; Lu, L.; Mase, K.; Relich, M.; Yoshida, S.] Southern Univ, Dept Phys, Baton Rouge, LA 70813 USA. [Gallagher, J.] Univ Wisconsin, Dept Astron, Madison, WI 53706 USA. [Hansen, E.; Koskinen, D. J.; Larson, M. J.; Medici, M.; Sarkar, S.] Univ Copenhagen, Niels Bohr Inst, DK-2100 Copenhagen, Denmark. [Homeier, A.; Voge, M.] Univ Bonn, Phys Inst, Nussallee 12, D-53115 Bonn, Germany. [Hoshina, K.] Univ Tokyo, Earthquake Res Inst, Bunkyo Ku, Tokyo 1130032, Japan. [Japaridze, G. S.] Clark Atlanta Univ, CTSPS, Atlanta, GA 30314 USA. [Kauer, M.; Maruyama, R.] Yale Univ, Dept Phys, New Haven, CT 06520 USA. [Kiryluk, J.; Lesiak-Bzdak, M.; Niederhausen, H.; Xu, Y.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Kohnen, G.] Univ Mons, B-7000 Mons, Belgium. [Kurahashi, N.; Richman, M.; Wills, L.] Drexel Univ, Dept Phys, Philadelphia, PA 19104 USA. [Madsen, J.; Seunarine, S.; Spiczak, G. M.] Univ Wisconsin, Dept Phys, River Falls, WI 54022 USA. [Palczewski, T.; Pepper, J. A.; Toale, P. A.; Williams, D. R.] Univ Alabama, Dept Phys & Astron, Tuscaloosa, AL 35487 USA. [Rawlins, K.] Univ Alaska Anchorage, Dept Phys & Astron, 3211 Providence Dr, Anchorage, AK 99508 USA. [Sarkar, S.] Univ Oxford, Dept Phys, 1 Keble Rd, Oxford OX1 3NP, England. [Sarkar, S.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. RP Aartsen, MG (reprint author), Univ Adelaide, Dept Phys, Adelaide, SA 5005, Australia. RI Tjus, Julia/G-8145-2012; Maruyama, Reina/A-1064-2013; Anton, Gisela/C-4840-2013; Beatty, James/D-9310-2011; Katz, Uli/E-1925-2013; Wiebusch, Christopher/G-6490-2012; Sarkar, Subir/G-5978-2011; Koskinen, David/G-3236-2014; OI Maruyama, Reina/0000-0003-2794-512X; Anton, Gisela/0000-0003-2039-4724; Beatty, James/0000-0003-0481-4952; Katz, Uli/0000-0002-7063-4418; Wiebusch, Christopher/0000-0002-6418-3008; Sarkar, Subir/0000-0002-3542-858X; Koskinen, David/0000-0002-0514-5917; Perez de los Heros, Carlos/0000-0002-2084-5866 FU U.S. National Science Foundation-Office of Polar Programs; U.S. National Science Foundation-Physics Division; University of Wisconsin Alumni Research Foundation; Grid Laboratory Of Wisconsin (GLOW) grid infrastructure at the University of Wisconsin Madison; Open Science Grid (OSG) grid infrastructure; U.S. Department of Energy; National Energy Research Scientific Computing Center; Louisiana Optical Network Initiative (LONI) grid computing resources; Natural Sciences and Engineering Research Council of Canada; WestGrid and Compute/Calcul Canada; Swedish Research Council; Swedish Polar Research Secretariat; Swedish National Infrastructure for Computing (SNIC); Knut and Alice Wallenberg Foundation, Sweden; German Ministry for Education and Research (BMBF); Deutsche Forschungsgemeinschaft (DFG); Helmholtz Alliance for Astroparticle Physics (HAP); Research Department of Plasmas with Complex Interactions (Bochum), Germany; Fund for Scientific Research (FNRS-FWO); FWO Odysseus programme; Flanders Institute to encourage scientific and technological research in industry (IWT); Belgian Federal Science Policy Office (Belspo); University of Oxford, United Kingdom; Marsden Fund, New Zealand; Australian Research Council; Japan Society for Promotion of Science (JSPS); Swiss National Science Foundation (SNSF), Switzerland; National Research Foundation of Korea (NRF); Villum Fonden, Danish National Research Foundation (DNRF), Denmark FX We acknowledge the support from the following agencies: U.S. National Science Foundation-Office of Polar Programs, U.S. National Science Foundation-Physics Division, University of Wisconsin Alumni Research Foundation, the Grid Laboratory Of Wisconsin (GLOW) grid infrastructure at the University of Wisconsin Madison, the Open Science Grid (OSG) grid infrastructure; U.S. Department of Energy, and National Energy Research Scientific Computing Center, the Louisiana Optical Network Initiative (LONI) grid computing resources; Natural Sciences and Engineering Research Council of Canada, WestGrid and Compute/Calcul Canada; Swedish Research Council, Swedish Polar Research Secretariat, Swedish National Infrastructure for Computing (SNIC), and Knut and Alice Wallenberg Foundation, Sweden; German Ministry for Education and Research (BMBF), Deutsche Forschungsgemeinschaft (DFG), Helmholtz Alliance for Astroparticle Physics (HAP), Research Department of Plasmas with Complex Interactions (Bochum), Germany; Fund for Scientific Research (FNRS-FWO), FWO Odysseus programme, Flanders Institute to encourage scientific and technological research in industry (IWT), Belgian Federal Science Policy Office (Belspo); University of Oxford, United Kingdom; Marsden Fund, New Zealand; Australian Research Council; Japan Society for Promotion of Science (JSPS); the Swiss National Science Foundation (SNSF), Switzerland; National Research Foundation of Korea (NRF); Villum Fonden, Danish National Research Foundation (DNRF), Denmark. NR 42 TC 3 Z9 3 U1 2 U2 3 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 2041-8205 EI 2041-8213 J9 ASTROPHYS J LETT JI Astrophys. J. Lett. PD JUN 20 PY 2016 VL 824 IS 2 AR L28 DI 10.3847/2041-8205/824/2/L28 PG 8 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DP0GU UT WOS:000378168200012 ER PT J AU McCann, BW De Silva, N Windus, TL Gordon, MS Moyer, BA Bryantsev, VS Hay, BP AF McCann, Billy W. De Silva, Nuwan Windus, Theresa L. Gordon, Mark S. Moyer, Bruce A. Bryantsev, Vyacheslav S. Hay, Benjamin P. TI Computer-Aided Molecular Design of Bis-phosphine Oxide Lanthanide Extractants SO INORGANIC CHEMISTRY LA English DT Article ID RARE-EARTH-ELEMENTS; MM3 FORCE-FIELD; CAMBRIDGE STRUCTURAL DATABASE; SOLVATION FREE-ENERGIES; NORMAL-BUTYL PHOSPHATE; CHELATE RING SIZE; SOLVENT-EXTRACTION; METAL-IONS; AQUEOUS-SOLUTION; VIBRATIONAL FREQUENCIES AB Computer-aided molecular design and high-throughput screening of viable host architectures can significantly reduce the efforts in the design of novel ligands for efficient extraction of rare earth elements. This paper presents a computational approach to the deliberate design of bis-phosphine oxide host architectures that are structurally organized for complexation of trivalent lanthanides. Molecule building software, HostDesigner, was interfaced with molecular mechanics software, PCModel, providing a tool for generating and screening millions of potential R-2(O)P-link-P(O)R-2 ligand geometries. The molecular mechanics ranking of ligand structures is consistent with both the solution-phase free energies of complexation obtained with density functional theory and the performance of known bis-phosphine oxide extractants. For the case where the link is -CH2-, evaluation of the ligand geometry provides the first characterization of a steric origin for the,`anomalous aryl strengthening" effect. The design approach has identified a number of novel bis-phosphine oxide ligands that are better organized for lanthanide complexation than previously studied examples. C1 [McCann, Billy W.; Moyer, Bruce A.; Bryantsev, Vyacheslav S.] Oak Ridge Natl Lab, Div Chem Sci, 1 Bethel Valley Rd, Oak Ridge, TN 37331 USA. [De Silva, Nuwan; Windus, Theresa L.; Gordon, Mark S.] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. [De Silva, Nuwan; Windus, Theresa L.; Gordon, Mark S.] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. [Hay, Benjamin P.] Supramol Design Inst, 127 Chestnut Hill Rd, Oak Ridge, TN 37830 USA. RP Bryantsev, VS (reprint author), Oak Ridge Natl Lab, Div Chem Sci, 1 Bethel Valley Rd, Oak Ridge, TN 37331 USA.; Hay, BP (reprint author), Supramol Design Inst, 127 Chestnut Hill Rd, Oak Ridge, TN 37830 USA. EM bryantsevv@ornl.gov; hayben@comcast.net RI Moyer, Bruce/L-2744-2016; Bryantsev, Vyacheslav/M-5111-2016 OI Moyer, Bruce/0000-0001-7484-6277; Bryantsev, Vyacheslav/0000-0002-6501-6594 FU Critical Materials Institute, an Energy Innovation Hub - U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Advanced Manufacturing Office; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Critical Materials Institute, an Energy Innovation Hub funded by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Advanced Manufacturing Office. This research used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The authors thank Drs. Marilu Dick-Perez and Federico Zahariev for helpful discussions. NR 99 TC 0 Z9 0 U1 10 U2 15 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD JUN 20 PY 2016 VL 55 IS 12 BP 5787 EP 5803 DI 10.1021/acs.inorgchem.5b02995 PG 17 WC Chemistry, Inorganic & Nuclear SC Chemistry GA DP3CL UT WOS:000378369900014 PM 26883005 ER PT J AU Cho, H Hong, K Strader, ML Lee, JH Schoenlein, RW Huse, N Kim, TK AF Cho, Hana Hong, Kiryong Strader, Matthew L. Lee, Jae Hyuk Schoenlein, Robert W. Huse, Nils Kim, Tae Kyu TI Electronic and Molecular Structure of the Transient Radical Photocatalyst Mn(CO)(5) and Its Parent Compound Mn-2(CO)(10) SO INORGANIC CHEMISTRY LA English DT Article ID RAY-ABSORPTION-SPECTROSCOPY; DENSITY-FUNCTIONAL CALCULATIONS; METAL-METAL BONDS; 2-DIMENSIONAL INFRARED-SPECTROSCOPY; EXPERIMENTAL CHARGE-DENSITY; MN-MN BOND; DIMANGANESE DECACARBONYL; K-EDGE; METHYL ACRYLATE; EXCITED-STATES AB We present a time-resolved X-ray spectroscopic study of the structural and electronic rearrangements of the photocatalyst Mn-2(CO)(10) upon photodeavage of the metal-metal bond. Our study of the manganese K-edge fine structure reveals details of both the molecular structure and valence charge distribution of the photodissociated radical product. Transient X-ray absorption spectra of the formation of the Mn(CO)(5) radical demonstrate surprisingly small structural modifications between the parent molecule and the resulting two identical manganese monomers. Small modifications of the local valence charge distribution are decisive for the catalytic activity of the radical product. The spectral changes reflect altered hybridization of metal-3d, metal-4p, and ligand-2p orbitals, particularly loss of interligand interaction, accompanied by the necessary spin transition due to radical formation. The spectral changes in the manganese pre- and main-edge region are well-reproduced by time-dependent density functional theory and ab initio multiple scattering calculations. C1 [Cho, Hana; Hong, Kiryong; Kim, Tae Kyu] Pusan Natl Univ, Dept Chem, Busan 46241, South Korea. [Cho, Hana; Hong, Kiryong; Strader, Matthew L.; Lee, Jae Hyuk; Schoenlein, Robert W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Ultrafast Xray Sci Lab, Berkeley, CA 94720 USA. [Huse, Nils] Univ Hamburg, Dept Phys, Max Planck Inst Struct & Dynam Matter, D-22761 Hamburg, Germany. [Huse, Nils] Ctr Free Electron Laser Sci, D-22761 Hamburg, Germany. [Cho, Hana] Korea Res Inst Stand & Sci, Ctr Inorgan Anal, Div Metrol Qual Life, Daejeon 34113, South Korea. [Strader, Matthew L.] SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Light Source, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. [Hong, Kiryong; Schoenlein, Robert W.] SLAC Natl Accelerator Lab, PULSE Inst, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. [Schoenlein, Robert W.] SLAC Natl Accelerator Lab, Linac Coherent Light Source, Menlo Pk, CA 94025 USA. RP Kim, TK (reprint author), Pusan Natl Univ, Dept Chem, Busan 46241, South Korea.; Schoenlein, RW (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Ultrafast Xray Sci Lab, Berkeley, CA 94720 USA.; Huse, N (reprint author), Univ Hamburg, Dept Phys, Max Planck Inst Struct & Dynam Matter, D-22761 Hamburg, Germany.; Huse, N (reprint author), Ctr Free Electron Laser Sci, D-22761 Hamburg, Germany.; Schoenlein, RW (reprint author), SLAC Natl Accelerator Lab, PULSE Inst, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA.; Schoenlein, RW (reprint author), SLAC Natl Accelerator Lab, Linac Coherent Light Source, Menlo Pk, CA 94025 USA. EM rwschoen@slac.stanford.edu; nils.huse@uni-hamburg.de; taim@pusan.ac.kr RI Huse, Nils/A-5712-2017 OI Huse, Nils/0000-0002-3281-7600 FU Office of Science, Office of Basic Energy Sciences, the Chemical Sciences, Geosciences, and Biosciences Division under the Department of Energy [DE-AC02-05CH11231]; National Research Foundation of Korea (NRF); Korean government (MEST) [2013S1A2A2035406, 2013R1A1A2009575, 2014R1A4A1001690]; Korean government (MSIP) [2013S1A2A2035406, 2013R1A1A2009575, 2014R1A4A1001690]; Max Planck POSTECH/Korea Research Initiative Program through the National Research Foundation of Korea (NRF) - Ministry of Science, ICT & Future Planning [2011-0031558]; Max Planck Society; City of Hamburg FX This research was supported by the Director, Office of Science, Office of Basic Energy Sciences, the Chemical Sciences, Geosciences, and Biosciences Division under the Department of Energy, Contract No. DE-AC02-05CH11231 (H.C, M.L.S, J.H.L, and R.W.S.) Experiments were conducted at the Advanced Light Source (LBNL), a DOE Office of Science User Facility. This work was supported by National Research Foundation of Korea (NRF) grants, funded by the Korean government (MEST and MSIP) (2013S1A2A2035406, 2013R1A1A2009575, and 2014R1A4A1001690). This work was also supported by Max Planck POSTECH/Korea Research Initiative Program [Grant 2011-0031558] through the National Research Foundation of Korea (NRF) funded by Ministry of Science, ICT & Future Planning. N.H. acknowledges funding from the Max Planck Society and the City of Hamburg. NR 79 TC 0 Z9 0 U1 11 U2 14 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD JUN 20 PY 2016 VL 55 IS 12 BP 5895 EP 5903 DI 10.1021/acs.inorgchem.6b00208 PG 9 WC Chemistry, Inorganic & Nuclear SC Chemistry GA DP3CL UT WOS:000378369900025 PM 27248860 ER PT J AU Ojwang, DO Grins, J Wardecki, D Valvo, M Renman, V Haggstrom, L Ericsson, T Gustafsson, T Mahmoud, A Hermann, RP Svensson, G AF Ojwang, Dickson O. Grins, Jekabs Wardecki, Dariusz Valvo, Mario Renman, Viktor Haggstrom, Lennart Ericsson, Tore Gustafsson, Torbjorn Mahmoud, Abdelfattah Hermann, Raphael P. Svensson, Gunnar TI Structure Characterization and Properties of K-Containing Copper Hexacyanoferrate SO INORGANIC CHEMISTRY LA English DT Article ID PRUSSIAN BLUE ANALOGS; INDUCED ELECTRON-TRANSFER; X-RAY-DIFFRACTION; SINGLE-CRYSTAL; ION BATTERIES; VIBRATIONAL-SPECTRA; MAGNETIC-PROPERTIES; PAINT LAYERS; CYANIDE; VACANCIES AB Copper hexacyanoferrate, Cu-II[Fe-III(CN)(6)](2/3)center dot nH(2)O, was synthesized, and varied amounts of IC ions were inserted via reduction by K2S2O3 (aq). Ideally, the reaction can be written as Cu-II[Fe-III(CN)(6)](2/3)-nH(2)O + 2x/3K(+) + 2x/3e(-)K(+) <-> K-2x/3 Cu-II[Fe-x(II).Fe-1-x(II),(CN)(6)](2/3)-nH(2)O. Infrared, Raman, and Mossbauer spectroscopy studies show that Fe-II is continuously reduced to Fell with increasing x, accompanied by a decrease of the a-axis of the cubic Fn (3) over barm unit cell. Elemental analysis of K by inductively coupled plasma shows that the insertion only begins when a significant fraction similar to 10% of the Fe-III, has already been reduced. Thermogravimetric analysis shows a fast exchange of water with ambient atmosphere and a total weight loss of similar to 26 wt % upon heating to 180 degrees C, above which the structure starts to decompose. The crystal structures of Cu-III[Fe-III(CN)(6)](2/3)center dot nH(2)O and K2/3Cu[Fe(CN)(6)](2/3)center dot nH(2)O were refined using synchrotron X-ray powder diffraction data. In both, one-third of the Fe(CN)(6) groups are vacant, and the octahedron around Cull is completed by water molecules. In the two structures, difference Fourier maps reveal three additional zeolitic water sites (8c, 32f, and 48g) in the center of the cavities formed by the-Cu-N-C-Fe- framework. The K-containing compound shows an increased electron density at two of these sites (32f and 48g), indicating them to be the preferred positions for the K+ ions. C1 [Ojwang, Dickson O.; Grins, Jekabs; Wardecki, Dariusz; Svensson, Gunnar] Stockholm Univ, Arrhenius Lab, Dept Mat & Environm Chem, SE-10691 Stockholm, Sweden. [Valvo, Mario; Renman, Viktor; Haggstrom, Lennart; Ericsson, Tore; Gustafsson, Torbjorn] Uppsala Univ, Angstrom Lab, Dept Chem, Box 538, SE-75121 Uppsala, Sweden. [Mahmoud, Abdelfattah; Hermann, Raphael P.] Forschungszentrum Julich, JARA FIT, Julich Ctr Neutron Sci JCNS, D-52425 Julich, Germany. [Mahmoud, Abdelfattah; Hermann, Raphael P.] Forschungszentrum Julich, JARA FIT, Peter Grunberg Inst PGI, D-52425 Julich, Germany. [Hermann, Raphael P.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Mahmoud, Abdelfattah] Univ Liege, Inst Phys, Inst Chem B63APTIS, LCIS GREENMAT, B-4000 Liege, Belgium. RP Svensson, G (reprint author), Stockholm Univ, Arrhenius Lab, Dept Mat & Environm Chem, SE-10691 Stockholm, Sweden. EM gunnar.svensson@mmk.su.se RI Hermann, Raphael/F-6257-2013; OI Hermann, Raphael/0000-0002-6138-5624; Ojwang, Dickson/0000-0001-9304-8975 FU "Consortium for Crystal Chemistry, C3" within Rontgen Angstrom duster, Swedish Research Council VR; Materials Sciences and Engineering Division, Office of Basic Energy Sciences, U.S. Department of Energy FX The authors acknowledge the "Consortium for Crystal Chemistry, C3" within the Rontgen Angstrom duster, Swedish Research Council VR, for providing financial support. R.P.H. acknowledges support from the Materials Sciences and Engineering Division, Office of Basic Energy Sciences, U.S. Department of Energy. We appreciate valuable comments from Prof. J. Mink, Hungarian Academy of Sciences, Budapest, Hungary. NR 69 TC 2 Z9 2 U1 26 U2 39 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD JUN 20 PY 2016 VL 55 IS 12 BP 5924 EP 5934 DI 10.1021/acs.inorgchem.6b00227 PG 11 WC Chemistry, Inorganic & Nuclear SC Chemistry GA DP3CL UT WOS:000378369900028 PM 27258790 ER PT J AU Zhu, JL Wang, YG Li, S Howard, JW Neuefeind, J Ren, Y Wang, H Liang, CD Yang, WG Zou, RQ Jin, CQ Zhao, YS AF Zhu, Jinlong Wang, Yonggang Li, Shuai Howard, John W. Neuefeind, Jorg Ren, Yang Wang, Hui Liang, Chengdu Yang, Wenge Zou, Ruqiang Jin, Changqing Zhao, Yusheng TI Sodium Ion Transport Mechanisms in Antiperovskite Electrolytes Na3OBr and Na4OI2: An in Situ Neutron Diffraction Study SO INORGANIC CHEMISTRY LA English DT Article ID ENERGY-STORAGE; SUPERIONIC CONDUCTORS; BATTERIES; CONDUCTIVITY; LI3OCL; LI; NA; CHALLENGES; STABILITY; CHEMISTRY AB Na-rich antiperovskites are recently developed solid electrolytes with enhanced sodium ionic conductivity and show promising functionality as a novel solid electrolyte in an all solid-state battery. In this work, the sodium ionic transport pathways of the parent compound Na3OBr, as well as the modified layered antiperovskite Na4OI2, were studied and compared through temperature-dependent neutron diffraction combined with the maximum entropy method. In the cubic Na30Br antiperovskite, the nuclear density distribution maps at SOO K indicate that sodium ions hop within and among oxygen octahedra, and Br- ions are not involved. In the tetragonal Na4OI2 antiperovskite, Na ions, which connect octahedra in the oh plane, have the lowest activation energy barrier. The transport of sodium ions along the c axis is assisted by I- ions. C1 [Zhu, Jinlong; Wang, Yonggang; Li, Shuai; Howard, John W.; Zhao, Yusheng] Univ Nevada, High Pressure Sci & Engn Ctr, Las Vegas, NV 89154 USA. [Wang, Yonggang] Carnegie Inst Sci, Geophys Lab, High Pressure Synerget Consortium, Argonne, IL 60439 USA. [Wang, Yonggang] Huanghe Sci & Technol Coll, Inst Nanostruct Funct Mat, Zhengzhou 450006, Henan, Peoples R China. [Neuefeind, Jorg] Oak Ridge Natl Lab, Neutron Scattering Sci Directorate, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. [Ren, Yang] Argonne Natl Lab, Adv Photon Source, 9700 S Cass Ave, Argonne, IL 60439 USA. [Wang, Hui; Liang, Chengdu] Oak Ridge Natl Lab, Mat Sci & Technol Div, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Wang, Hui; Liang, Chengdu] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Yang, Wenge] Ctr High Pressure Sci & Technol Adv Res HPSTAR, Shanghai 201203, Peoples R China. [Zou, Ruqiang] Peking Univ, Beijing Key Lab Theory & Technol Adv Battery Mat, Coll Engn, Beijing 100871, Peoples R China. [Jin, Changqing] Chinese Acad Sci, Inst Phys, Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China. RP Zhao, YS (reprint author), Univ Nevada, High Pressure Sci & Engn Ctr, Las Vegas, NV 89154 USA.; Zou, RQ (reprint author), Peking Univ, Beijing Key Lab Theory & Technol Adv Battery Mat, Coll Engn, Beijing 100871, Peoples R China. EM rzou@pku.edu.cn; yusheng.zhao@unlv.edu OI Wang, Yonggang/0000-0003-4816-9182; Zou, Ruqiang/0000-0003-0456-4615 FU High Pressure Science and Engineering Center (HiPSEC), University of Nevada, Las Vegas; National Nuclear Security Administration under the Stewardship Science Academic Alliances program through DOE [DE-NA0001982]; Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy; NSF through Institute of Physics, Chinese Academy of Sciences; MOST of China through Institute of Physics, Chinese Academy of Sciences; DOE-BES X-ray Scattering Core Program [DE-FG02-99ER45775] FX We thank the High Pressure Science and Engineering Center (HiPSEC), University of Nevada, Las Vegas, for support. This research was sponsored in part by the National Nuclear Security Administration under the Stewardship Science Academic Alliances program through DOE Cooperative Agreement #DE-NA0001982. A portion of this research at ORNL's Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. We acknowledge the support from NSF & MOST of China through research projects at Institute of Physics, Chinese Academy of Sciences. W.Y. acknowledges the financial support from DOE-BES X-ray Scattering Core Program under Grant DE-FG02-99ER45775. NR 36 TC 0 Z9 0 U1 24 U2 55 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD JUN 20 PY 2016 VL 55 IS 12 BP 5993 EP 5998 DI 10.1021/acs.inorgchem.6b00444 PG 6 WC Chemistry, Inorganic & Nuclear SC Chemistry GA DP3CL UT WOS:000378369900034 PM 27251879 ER PT J AU Yu, RZ Matsuda, N Tominaga, K Shimizu, K Hojo, H Sakai, Y Yamamoto, H Oka, K Azuma, M AF Yu, Runze Matsuda, Narumi Tominaga, Ken Shimizu, Keisuke Hojo, Hajime Sakai, Yuki Yamamoto, Hajime Oka, Kengo Azuma, Masaki TI High-Temperature Monoclinic Cc Phase with Reduced c/a Ratio in Bi-based Perovskite Compound Bi2ZnTi1-xMnxO6 SO INORGANIC CHEMISTRY LA English DT Article ID HIGH-PRESSURE SYNTHESIS; POWDER DIFFRACTION; SOLID-SOLUTION; BOUNDARY; CERAMICS; TRANSITION; CRYSTAL; SYSTEM; BINIO3; PIEZOELECTRICITY AB Monoclinic phases with Cm, Pm, and Cc space groups are indispensable to understand the high performance of electromechanical properties at the morphotropic phase boundary (MPB) of lead-based perovskite oxides Pb (ZrxTi1-x)O-3 (PZT), [Pb (Mg1/3Nb2/3)O-3](1-x) (PbTiO3)(x) (PMN-PT), and [Pb(Zn1/3Nb2/3)O-3](1-x)-(PbTiO3)(x) (PZN-PT). Here, a nearly single monoclinic phase with space group Cc was observed in the Bi-based lead-free perovskite compound Bi2ZnTi1-xMnxO6 at x = 0.4. This phase was the same as the low-temperature phase of the MPB composition of PZT but existed at a much higher temperature. Despite the reduced pseudo c/a ratio of 1.065, which is the same as that of PbTiO3 at room temperature, ionic model calculation based on the Rietveld refinement data indicated the polarization of Bi2ZnTi0.6Mn0.4O6 is 95.8 mu C/cm(2). The tilting and significant anisotropic distortion of the octahedron were found to cause the c/a ratio to reduce. Accordingly, the effective piezoelectric constant d(33) of Bi2ZnTi0.6Mn0.4O6 thin film was found to be 12 pm/V. C1 [Yu, Runze; Matsuda, Narumi; Tominaga, Ken; Shimizu, Keisuke; Hojo, Hajime; Yamamoto, Hajime; Azuma, Masaki] Tokyo Inst Technol, Mat & Struct Lab, Midori Ku, 4259 Nagatsuta, Yokohama, Kanagawa 2268503, Japan. [Sakai, Yuki] Kanagawa Acad Sci & Technol, KSP, Takatsu Ku, 3-2-1 Sakado, Kawasaki, Kanagawa 2130012, Japan. [Oka, Kengo] Chuo Univ, Fac Sci & Engn, Dept Appl Chem, Bunkyo Ku, 1-13-27 Kasuga, Tokyo 1128551, Japan. [Yu, Runze] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RP Hojo, H; Azuma, M (reprint author), Tokyo Inst Technol, Mat & Struct Lab, Midori Ku, 4259 Nagatsuta, Yokohama, Kanagawa 2268503, Japan. EM hhojo@msl.titech.ac.jp; mazuma@msl.titech.ac.jp RI Oka, Kengo/A-8753-2010; Hojo, Hajime/C-5275-2012 OI Oka, Kengo/0000-0002-1800-8575; FU Japan Society for the Promotion of Science (JSPS) [26106507, 26820291, 26800180, 15K14119]; Japan Synchrotron Radiation Research Institute [2014A1732, 2014A3615, 2014B1731, 2015A1788, 2015A3615, 2015B1730]; Shared User Program of JAEA Facilities [2014A-E21, 2015A -E11]; Ministry of Education, Culture, Sports, Science and Technology [A-14-AE-0015, A-15-AE-0011] FX Authors acknowledge J. Chen at Univ. of Science and Technology Beijing for fruitful discussions. This work was supported by the Scientific Research on Innovative Areas (26106507), Young Scientists (B) (26820291 and 26800180), and Challenging Exploratory Research (15K14119) from the Japan Society for the Promotion of Science (JSPS). The synchrotron -radiation experiments were performed at SPring-8 with the approval of the Japan Synchrotron Radiation Research Institute (2014A1732, 2014A3615, 2014B1731, 2015A1788, 2015A3615, and 2015B1730) and under the Shared User Program of JAEA Facilities (Grant Nos. 2014A-E21 and 2015A -E11) with the approval of the Nanotechnology Platform project supported by the Ministry of Education, Culture, Sports, Science and Technology (Grant Nos. A-14-AE-0015 and A-15-AE-0011). NR 43 TC 3 Z9 3 U1 6 U2 13 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD JUN 20 PY 2016 VL 55 IS 12 BP 6124 EP 6129 DI 10.1021/acs.inorgchem.6b00618 PG 6 WC Chemistry, Inorganic & Nuclear SC Chemistry GA DP3CL UT WOS:000378369900050 PM 27254112 ER PT J AU Gorne, AL George, J van Leusen, J Duck, G Jacobs, P Muniraju, NKC Dronskowski, R AF Goerne, Arno L. George, Janine van Leusen, Jan Dueck, Gerald Jacobs, Philipp Muniraju, Naveen Kumar Chogondahalli Dronskowski, Richard TI Ammonothermal Synthesis, Crystal Structure, and Properties of the Ytterbium(II) and Ytterbium(III) Amides and the First Two Rare-Earth-Metal Guanidinates, YbC(NH)(3) and Yb(CN3H4)(3) SO INORGANIC CHEMISTRY LA English DT Article ID BOND-VALENCE PARAMETERS; NEUTRON POWDER DIFFRACTION; AUGMENTED-WAVE METHOD; LIQUID-AMMONIA; TETRAPHENYLARSONIUM PENTAKIS(NITRATO)YTTERBATE(III); ELECTRONIC-STRUCTURE; COMPLEXES; LIGANDS; POTASSIUM; MAGNETISM AB We report the oxidation-controlled synthesis of the ytterbium amides Yb(NH2)(2) and Yb(NH2)(3) and the first rare-earth metal guanidinates YbC(NH2)(2), and Yb(CN3H4)(3) from liquid ammonia. For Yb(N1-12)2, we present experimental atomic displacement parameters from powder X-ray diffraction (PXRD) and density functional theory (DFT)-derived hydrogen positions for the first time. For Yb(NH2)(3), the indexing proposal based on PXRD arrives at R (3) over bar, a = 6.2477(2) angstrom, c = 17.132(1) angstrom, V = 579.15(4) angstrom(3), and Z = 6. The oxidation-controlled synthesis was also applied to make the first rare-earth guanidinates, namely, the doubly deprotonated YbC(NH)(3) and the singly deprotonated Yb(CN3H4)(3). YbC(NH)(3) is isostructural with SrC(NH)(3), as derived from PXRD (P6(3)/m, a = 5.2596(2) angstrom, c = 6.6704(2) angstrom, v = 159.81(1) angstrom(3), and Z = 2). Yb(CN3H4)(3) crystallizes in a structure derived from the [ReO3] type, as studied by powder neutron diffraction (Pn (3) over bar, a = 13.5307(3) angstrom, v = 2477.22(8) angstrom(3), and Z = 8 at 10 K). Electrostatic and hydrogen-bonding interactions cooperate to stabilize the structure with wide and empty channels. The IR spectra of the guanidinates are compared with DFT-calculated phonon spectra to identify the vibrational modes. SQUID magnetometry shows that Yb(CN3H4)(3) is a paramagnet with isolated Yb3+ (4f(13)) ions. A CONDON 2.0 fit was used to extract all relevant parameters. C1 [Goerne, Arno L.; George, Janine; van Leusen, Jan; Dueck, Gerald; Jacobs, Philipp; Dronskowski, Richard] Rhein Westfal TH Aachen, Inst Inorgan Chem, Landoltweg 1, D-52056 Aachen, Germany. [Muniraju, Naveen Kumar Chogondahalli] Forschungszentrum Julich, JCNS, Outstn Spallat Neutron Source SNS, Oak Ridge, TN 37831 USA. [Muniraju, Naveen Kumar Chogondahalli] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. RP Dronskowski, R (reprint author), Rhein Westfal TH Aachen, Inst Inorgan Chem, Landoltweg 1, D-52056 Aachen, Germany. EM drons@hal9000.ac.rwth-aachen.de OI Chogondahalli Muniraju, Naveen Kumar/0000-0002-8867-8291 FU JCNS; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; Fonds der Chemischen Industrie; JARA-HPC from RWTH Aachen University [JARA0069] FX We thank Paul Muller for PXRD measurements, Christina Houben for SQUID magnetometry measurements, and Melanie Kirkham for assistance with the neutron diffraction experiments at POWGEN. The authors gratefully acknowledge the financial support provided by JCNS to perform the neutron scattering measurements at the SNS, Oak Ridge, TN. Part of the research conducted at the SNS was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. Moreover, J.G. thanks the Fonds der Chemischen Industrie for a scholarship. DFT calculations were performed with computing resources thankfully granted by JARA-HPC from RWTH Aachen University under Project JARA0069. NR 75 TC 0 Z9 0 U1 8 U2 18 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD JUN 20 PY 2016 VL 55 IS 12 BP 6161 EP 6168 DI 10.1021/acs.inorgchem.6b00736 PG 8 WC Chemistry, Inorganic & Nuclear SC Chemistry GA DP3CL UT WOS:000378369900054 PM 27248288 ER PT J AU Nguyen, NTT Lo, TNH Kim, J Nguyen, HTD Le, TB Cordova, KE Furukawa, H AF Nguyen, Nhung T. T. Lo, Tien N. H. Kim, Jaheon Nguyen, Huong T. D. Le, Toan B. Cordova, Kyle E. Furukawa, Hiroyasu TI Mixed-Metal Zeolitic Imidazolate Frameworks and their Selective Capture of Wet Carbon Dioxide over Methane SO INORGANIC CHEMISTRY LA English DT Article ID ORGANIC FRAMEWORKS; CO2 CAPTURE; CRYSTAL; WATER; ADSORPTION; SEPARATION; STABILITY; CLUSTERS; DESIGN; SITES AB A presynthesized, square planar copper imidazole complex, [Cu(imidazole)(4)](NO3)(2), was utilized as a precursor in the synthesis of a new series of zeolitic imidazolate frameworks, termed ZIF-202, -203, and -204. The structures of all three members were solved by single-crystal X-ray diffraction analysis, which revealed ZIF-203 and -204 having successfully integrated square planar units within the backbones of their respective frameworks. As a result of this unit, the structures of both ZIF-203 and -204 were found to adopt unprecedented three-dimensional nets, namely, ntn and thl, respectively. One member of this series, ZIF-204, was demonstrated to be highly porous, exhibit exceptional stability in water, and selectively capture CO2 over CH4 under both dry and wet conditions without any loss in performance over three cycles. Remarkably, the regeneration of ZIF-204 was performed under the mild conditions of flowing a pure N-2 gas through the material at ambient temperature. C1 [Nguyen, Nhung T. T.; Lo, Tien N. H.; Nguyen, Huong T. D.; Le, Toan B.] Vietnam Natl Univ Ho Chi Minh City, Univ Sci, Fac Chem, Ho Chi Minh City 721337, Vietnam. [Nguyen, Nhung T. T.; Le, Toan B.] Can Tho Univ, Sch Educ, Dept Chem, Can Tho City 721337, Vietnam. [Kim, Jaheon] Soongsil Univ, Dept Chem, 369 Sangdo Ro, Seoul 156743, South Korea. [Cordova, Kyle E.; Furukawa, Hiroyasu] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Dept Chem, Berkeley, CA 94720 USA. [Cordova, Kyle E.; Furukawa, Hiroyasu] Berkeley Global Sci Inst, Berkeley, CA 94720 USA. [Cordova, Kyle E.; Furukawa, Hiroyasu] King Fahd Univ Petr & Minerals, Ctr Res Excellence Nanotechnol, Dhahran 34464, Saudi Arabia. RP Cordova, KE; Furukawa, H (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Dept Chem, Berkeley, CA 94720 USA.; Cordova, KE; Furukawa, H (reprint author), Berkeley Global Sci Inst, Berkeley, CA 94720 USA.; Cordova, KE; Furukawa, H (reprint author), King Fahd Univ Petr & Minerals, Ctr Res Excellence Nanotechnol, Dhahran 34464, Saudi Arabia. EM kcordova@berkeley.edu; furukawa@berkeley.edu OI Cordova, Kyle/0000-0002-4988-0497 FU VNU-HCM [A2015-50-01-HD-KHCN]; United States Office of Naval Research Global: Naval International Cooperative Opportunities in Science and Technology Program [N62909-15-1N056] FX Financial support for the synthesis, characterization, and gas adsorption measurements were provided by VNU-HCM (A2015-50-01-HD-KHCN) and the United States Office of Naval Research Global: Naval International Cooperative Opportunities in Science and Technology Program (No. N62909-15-1N056). NR 46 TC 0 Z9 0 U1 15 U2 38 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD JUN 20 PY 2016 VL 55 IS 12 BP 6201 EP 6207 DI 10.1021/acs.inorgchem.6b00814 PG 7 WC Chemistry, Inorganic & Nuclear SC Chemistry GA DP3CL UT WOS:000378369900059 PM 27248714 ER PT J AU Jentzen, W Shelnutt, JA Scheidt, WR AF Jentzen, Walter Shelnutt, John A. Scheidt, W. Robert TI Metalloporphines: Dimers and Trimers SO INORGANIC CHEMISTRY LA English DT Article ID LIGHT-ABSORPTION PROPERTIES; MOLECULAR-STRUCTURE; SOLID-STATE; PHOTOSYNTHETIC CHROMOPHORES; CRYSTAL-STRUCTURE; NICKEL(II); PORPHINE; PORPHYRINS; STEREOCHEMISTRY; COMPLEXES AB Procedures for the purification and subsequent crystallization of the slightly soluble four-coordinate metal-porphines, the simplest possible porphyrin derivatives, are described. Crystals of the porphine derivatives of cobalt(II), copper(II), platinum(II), and two polymorphs of zinc(II) were obtained. Analysis of the crystal and molecular structures shows that all except the platinum(II) derivative form an unusual trimeric species in the solid state. The isomorphous cobalt(II), copper(II), and one zinc(II) polymorph pack in the unit cell to form dimers as well as the trimers. Interplanar spacings between porphine rings are similar in both the dimers and trimers and range between 3.24 and 3.37 angstrom. Porphine rings are strongly overlapped with lateral shifts between ring centers in both the dimers and trimers with values between 1.52 and 1.70 angstrom or in Category S as originally defined by Scheidt and Lee. Periodic trends in the M-N-P bond distances parallel those observed previously for tetraphenyl- and ctaethylporphyrin derivatives. C1 [Jentzen, Walter] Sandia Natl Labs, Fuel Sci Dept, POB 5800, Albuquerque, NM 87185 USA. [Shelnutt, John A.] Univ New Mexico, Dept Chem, Albuquerque, NM 87131 USA. [Scheidt, W. Robert] Univ Notre Dame, Dept Chem & Biochem, Notre Dame, IN 46556 USA. [Jentzen, Walter] Univ Duisburg Essen, Univ Hosp Essen, Dept Nucl Med, Hufelandstr 55, D-45122 Essen, Germany. RP Jentzen, W (reprint author), Sandia Natl Labs, Fuel Sci Dept, POB 5800, Albuquerque, NM 87185 USA.; Scheidt, WR (reprint author), Univ Notre Dame, Dept Chem & Biochem, Notre Dame, IN 46556 USA.; Jentzen, W (reprint author), Univ Duisburg Essen, Univ Hosp Essen, Dept Nucl Med, Hufelandstr 55, D-45122 Essen, Germany. EM walter.jentzen@uni-due.de; scheidt.1@nd.edu FU National Institutes of Health [GM-38401] FX Research reported in this publication was supported by the National Institutes of Health under Grant GM-38401 to W.R.S. We thank Dr. Mayou Shang for technical assistance with the Xray structure determinations. NR 49 TC 0 Z9 0 U1 6 U2 14 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD JUN 20 PY 2016 VL 55 IS 12 BP 6294 EP 6299 DI 10.1021/acs.inorgchem.6b00956 PG 6 WC Chemistry, Inorganic & Nuclear SC Chemistry GA DP3CL UT WOS:000378369900070 PM 27276239 ER PT J AU Gamel, O AF Gamel, Omar TI Entangled Bloch spheres: Bloch matrix and two-qubit state space SO PHYSICAL REVIEW A LA English DT Article ID N-LEVEL SYSTEMS; MIXED STATES; DENSITY-MATRICES; SEPARABILITY; PARAMETERS; GEOMETRY; VECTOR AB We represent a two-qubit density matrix in the basis of Pauli matrix tensor products, with the coefficients constituting a Bloch matrix, analogous to the single qubit Bloch vector. We find the quantum state positivity requirements on the Bloch matrix components, leading to three important inequalities, allowing us to parametrize and visualize the two-qubit state space. Applying the singular value decomposition naturally separates the degrees of freedom to local and nonlocal, and simplifies the positivity inequalities. It also allows us to geometrically represent a state as two entangled Bloch spheres with superimposed correlation axes. It is shown that unitary transformations, local or nonlocal, have simple interpretations as axis rotations or mixing of certain degrees of freedom. The nonlocal unitary invariants of the state are then derived in terms of local unitary invariants. The positive partial transpose criterion for entanglement is generalized, and interpreted as a reflection, or a change of a single sign. The formalism is used to characterize maximally entangled states, and generalize two qubit isotropic and Werner states. C1 [Gamel, Omar] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Gamel, Omar] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Gamel, O (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Gamel, O (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. EM ogamel@berkeley.edu FU Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; Division of Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Sciences [DE-AC03-76F000098] FX I thank Prof. Graham Fleming for his support and for proposing research problems that motivated this manuscript. I also thank Prof. Birgitta Whaley for bringing to my attention several important references, and the anonymous referees for valuable suggestions. This work was supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231 and the Division of Chemical Sciences, Geosciences and Biosciences Division, Office of Basic Energy Sciences through Grant No. DE-AC03-76F000098 (at LBNL and UC Berkeley). NR 53 TC 3 Z9 3 U1 2 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9926 EI 2469-9934 J9 PHYS REV A JI Phys. Rev. A PD JUN 20 PY 2016 VL 93 IS 6 AR 062320 DI 10.1103/PhysRevA.93.062320 PG 18 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA DO9JZ UT WOS:000378103800002 ER PT J AU Ozer, ZN Ali, E Dogan, M Yavuz, M Alwan, O Naja, A Chuluunbaatar, O Joulakian, BB Ning, CG Colgan, J Madison, D AF Ozer, Zehra N. Ali, Esam Dogan, Mevlut Yavuz, Murat Alwan, Osman Naja, Adnan Chuluunbaatar, Ochbadrakh Joulakian, Boghos B. Ning, Chuan-Gang Colgan, James Madison, Don TI Comparison of experimental and theoretical triple differential cross sections for the single ionization of CO2 (1 pi(g)) by electron impact SO PHYSICAL REVIEW A LA English DT Article ID CARBON-DIOXIDE; COLLISIONS; EXCITATION; ORBITALS; STATES; GASES; H2O AB Experimental and theoretical triple differential cross sections for intermediate-energy (250 eV) electron-impact single ionization of the CO2 are presented for three fixed projectile scattering angles. Results are presented for ionization of the outermost 1 pi(g) molecular orbital of CO2 in a coplanar asymmetric geometry. The experimental data are compared to predictions from the three-center Coulomb continuum approximation for triatomic targets, and the molecular three-body distorted wave (M3DW) model. It is observed that while both theories are in reasonable qualitative agreement with experiment, the M3DW is in the best overall agreement with experiment. C1 [Ozer, Zehra N.; Dogan, Mevlut; Yavuz, Murat] Afyon Kocatepe Univ, Dept Phys, E COL Lab, TR-03200 Afyon, Turkey. [Ali, Esam; Madison, Don] Missouri Univ Sci & Technol, Dept Phys, Rolla, MO 65409 USA. [Alwan, Osman; Naja, Adnan] Lebanese Univ, LPM, EDST, Tripoli 1300, Lebanon. [Alwan, Osman; Joulakian, Boghos B.] Univ Lorraine, SRSMC, UMR CNRS 7565, 1 Bld Arago,Bat ICPM, F-57078 Metz 3, France. [Chuluunbaatar, Ochbadrakh] Joint Inst Nucl Res, Dubna 141980, Moscow Region, Russia. [Ning, Chuan-Gang] Tsinghua Univ, Dept Phys, State Key Lab Low Dimens Quantum Phys, Beijing 100084, Peoples R China. [Colgan, James] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Ozer, ZN (reprint author), Afyon Kocatepe Univ, Dept Phys, E COL Lab, TR-03200 Afyon, Turkey. EM zehraerengil@aku.edu.tr FU Scientific and Technological Research Council of Turkey (TUBITAK) [109T738]; BAPK [15.HIZ.DES.130, 14FENED.06]; US National Science Foundation [PHY-1505819]; National Natural Science Foundation of China [11174175]; National Nuclear Security Administration of the US Department of Energy [DE-AC5206NA25396] FX This work was supported by the Scientific and Technological Research Council of Turkey (TUBITAK) through Grant No. 109T738 and by BAPK through Grant No. 15.HIZ.DES.130, 14FENED.06. E.A. and D.M. would like to acknowledge the support of the US National Science Foundation under Grant. No. PHY-1505819 and C.N. would like to acknowledge the support of the National Natural Science Foundation of China under Grant No. 11174175. Computational work was performed with Institutional Computing resources made available through the Los Alamos National Laboratory. The Los Alamos National Laboratory is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the US Department of Energy under Contract No. DE-AC5206NA25396. NR 44 TC 0 Z9 0 U1 7 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9926 EI 2469-9934 J9 PHYS REV A JI Phys. Rev. A PD JUN 20 PY 2016 VL 93 IS 6 AR 062707 DI 10.1103/PhysRevA.93.062707 PG 6 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA DO9JZ UT WOS:000378103800009 ER PT J AU Aczel, AA Cook, AM Williams, TJ Calder, S Christianson, AD Cao, GX Mandrus, D Kim, YB Paramekanti, A AF Aczel, A. A. Cook, A. M. Williams, T. J. Calder, S. Christianson, A. D. Cao, G. -X. Mandrus, D. Kim, Yong-Baek Paramekanti, A. TI Highly anisotropic exchange interactions of j(eff)=1/2 iridium moments on the fcc lattice in La2BIrO6 (B = Mg, Zn) SO PHYSICAL REVIEW B LA English DT Article ID ORDERED DOUBLE PEROVSKITE; MAGNETIC-PROPERTIES; NEUTRON-DIFFRACTION; CSCOCL3; SCATTERING AB We have performed inelastic neutron scattering (INS) experiments to investigate the magnetic excitations in the weakly distorted face-centered-cubic (fcc) iridate double perovskites La2ZnIrO6 and La2MgIrO6, which are characterized by A-type antiferromagnetic ground states. The powder inelastic neutron scattering data on these geometrically frustrated j(eff) = 1/2 Mott insulators provide clear evidence for gapped spin-wave excitations with very weak dispersion. The INS results and thermodynamic data on these materials can be reproduced by conventional Heisenberg-Ising models with significant uniaxial Ising anisotropy and sizeable second-neighbor ferromagnetic interactions. Such a uniaxial Ising exchange interaction is symmetry forbidden on the ideal fcc lattice, so that it can only arise from the weak crystal distortions away from the ideal fcc limit. This may suggest that even weak distortions in j(eff) = 1/2 Mott insulators might lead to strong exchange anisotropies. More tantalizingly, however, we find an alternative viable explanation of the INS results in terms of spin models with a dominant Kitaev interaction. In contrast to the uniaxial Ising exchange, the highly directional Kitaev interaction is a type of exchange anisotropy which is symmetry allowed even on the ideal fcc lattice. The Kitaev model has a magnon gap induced by quantum order by disorder, while weak anisotropies of the Kitaev couplings generated by the symmetry lowering due to lattice distortions can pin the order and enhance the magnon gap. Our findings highlight how even conventional magnetic orders in heavy transition metal oxides may be driven by highly directional exchange interactions rooted in strong spin-orbit coupling. C1 [Aczel, A. A.; Williams, T. J.; Calder, S.; Christianson, A. D.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Cook, A. M.; Kim, Yong-Baek; Paramekanti, A.] Univ Toronto, Dept Phys, Toronto, ON M5S 1A7, Canada. [Cao, G. -X.; Mandrus, D.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Mandrus, D.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Kim, Yong-Baek; Paramekanti, A.] Canadian Inst Adv Res, Toronto, ON M5G 1Z8, Canada. RP Aczel, AA (reprint author), Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA.; Paramekanti, A (reprint author), Univ Toronto, Dept Phys, Toronto, ON M5S 1A7, Canada.; Paramekanti, A (reprint author), Canadian Inst Adv Res, Toronto, ON M5G 1Z8, Canada. EM aczelaa@ornl.gov; arunp@physics.utoronto.ca RI christianson, andrew/A-3277-2016 OI christianson, andrew/0000-0003-3369-5884 FU U.S. Department of Energy (DOE), Office of Basic Energy Sciences; Scientific User Facilities Division; Materials Science and Engineering Division; Wigner Fellowship program at ORNL; NSERC of Canada FX We thank M. D. Lumsden, S. E. Nagler, and K. W. Plumb for useful discussions and V. O. Garlea for technical support. This research was supported by the U.S. Department of Energy (DOE), Office of Basic Energy Sciences. Inelastic neutron scattering experiments were performed at the Spallation Neutron Source and the High Flux Isotope Reactor, which are sponsored by the Scientific User Facilities Division. A. A. A., S.C., and A.D.C. were supported by the Scientific User Facilities Division. G.-X.C. and D.M. were supported by the Materials Science and Engineering Division. T.J.W. acknowledges support from the Wigner Fellowship program at ORNL. A.M.C., Y.B.K., and A.P. were funded by NSERC of Canada. NR 78 TC 3 Z9 3 U1 11 U2 23 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUN 20 PY 2016 VL 93 IS 21 AR 214426 DI 10.1103/PhysRevB.93.214426 PG 11 WC Physics, Condensed Matter SC Physics GA DO9KB UT WOS:000378104000004 ER PT J AU Banerjee, S Agren, H Balatsky, AV AF Banerjee, Saikat Agren, Hans Balatsky, A. V. TI Landau-like states in neutral particles SO PHYSICAL REVIEW B LA English DT Article ID ELECTRIC-DIPOLE; SPIN; ATOMS AB We show the emergence of a new type of dispersion relation for neutral atoms with an interesting similarity to the spectrum of two-dimensional electrons in an applied perpendicular constant magnetic field. These neutral atoms can be confined in toroidal optical traps and give quasi-Landau spectra. In strong contrast to the equidistant infinitely degenerate Landau levels for charged particles, the spectral gap for such two-dimensional neutral particles increases in particular electric-field configurations. The idea in the paper is motivated by the development in cold atom experiments and builds on the seminal paper of Aharonov and Casher. C1 [Banerjee, Saikat; Balatsky, A. V.] Los Alamos Natl Lab, Inst Mat Sci, Los Alamos, NM 87545 USA. [Banerjee, Saikat; Balatsky, A. V.] KTH Royal Inst Technol, Nordita, Ctr Quantum Mat, Roslagstullsbacken 23, S-10691 Stockholm, Sweden. [Banerjee, Saikat; Balatsky, A. V.] Stockholm Univ, Roslagstullsbacken 23, S-10691 Stockholm, Sweden. [Banerjee, Saikat; Agren, Hans] Royal Inst Technol, Div Theoret Chem & Biol, SE-10691 Stockholm, Sweden. RP Banerjee, S (reprint author), Los Alamos Natl Lab, Inst Mat Sci, Los Alamos, NM 87545 USA.; Banerjee, S (reprint author), KTH Royal Inst Technol, Nordita, Ctr Quantum Mat, Roslagstullsbacken 23, S-10691 Stockholm, Sweden.; Banerjee, S (reprint author), Stockholm Univ, Roslagstullsbacken 23, S-10691 Stockholm, Sweden.; Banerjee, S (reprint author), Royal Inst Technol, Div Theoret Chem & Biol, SE-10691 Stockholm, Sweden. FU ERC Grant [DM 321031]; U.S. DOE Grant [BES E3B7]; Swedish Science Research Council [2012-3447]; Knut and Alice Wallenberg Foundation [KAW-2013.0020] FX S.B. is grateful to J. Larson, Stockholm University and E. Sjoqvist, Uppsala University for many important discussions regarding the idea of the paper and cold atomic experiments. This work was supported by ERC Grant No. DM 321031, U.S. DOE Grant No. BES E3B7, and by the Swedish Science Research Council (Grant No. 2012-3447). S.B. and H.A. acknowledge The Knut and Alice Wallenberg Foundation for financial support (Grant No. KAW-2013.0020). NR 27 TC 1 Z9 1 U1 2 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUN 20 PY 2016 VL 93 IS 23 AR 235134 DI 10.1103/PhysRevB.93.235134 PG 4 WC Physics, Condensed Matter SC Physics GA DO9KO UT WOS:000378105400001 ER PT J AU Coh, S Lee, DH Louie, SG Cohen, ML AF Coh, Sinisa Lee, Dung-Hai Louie, Steven G. Cohen, Marvin L. TI Proposal for a bulk material based on a monolayer FeSe on SrTiO3 high-temperature superconductor SO PHYSICAL REVIEW B LA English DT Article ID SINGLE-LAYER FESE; PHASE-DIAGRAM; PHOTOEMISSION-SPECTROSCOPY; STRONTIUM-TITANATE; ELECTRONIC ORIGIN; THIN-FILMS; 65 K; INSTABILITIES; PEROVSKITES AB Motivated by the high superconducting transition temperature of monolayer FeSe on SrTiO3, we propose a potential three-dimensional high-temperature superconductor superlattice FeSe-SrTiO3 and study its structural stability and electronic structure using density functional theory. We find that the binding energy between the FeSe and SrTiO3 layers is about similar to 0.7 eV per (Fe2Se2) unit and that it saturates already within a single TiO2 atomic layer of SrTiO3. In addition we analyzed the dynamical stability of the superlattice and compared it to the case of bulk SrTiO3. C1 [Coh, Sinisa] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Coh, S (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM sinisacoh@gmail.com FU Theory Program at the Lawrence Berkeley National Lab through the Office of Basic Energy Sciences, U.S. Department of Energy [DE-AC02-05CH11231]; National Science Foundation [DMR15-1508412]; Office of Science of the U.S. Department of Energy FX This work was supported by the Theory Program at the Lawrence Berkeley National Lab through the Office of Basic Energy Sciences, U.S. Department of Energy under Contract No. DE-AC02-05CH11231 which provided for the theoretical analysis and the National Science Foundation under Grant No. DMR15-1508412 which provided for the structural calculation. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy. NR 44 TC 2 Z9 2 U1 9 U2 22 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUN 20 PY 2016 VL 93 IS 24 AR 245138 DI 10.1103/PhysRevB.93.245138 PG 6 WC Physics, Condensed Matter SC Physics GA DO9KX UT WOS:000378106400003 ER PT J AU Jungfleisch, MB Zhang, W Sklenar, J Jiang, W Pearson, JE Ketterson, JB Hoffmann, A AF Jungfleisch, M. B. Zhang, W. Sklenar, J. Jiang, W. Pearson, J. E. Ketterson, J. B. Hoffmann, A. TI Interface-driven spin-torque ferromagnetic resonance by Rashba coupling at the interface between nonmagnetic materials SO PHYSICAL REVIEW B LA English DT Article ID INSULATOR AB The Rashba-Edelstein effect stems from the interaction between the electron's spin and its momentum induced by spin-orbit interaction at an interface or a surface. It was shown that the inverse Rashba-Edelstein effect can be used to convert a spin current into a charge current. Here, we demonstrate the reverse process of a charge-to spin-current conversion at a Bi/Ag Rashba interface. We show that this interface-driven spin current can drive an adjacent ferromagnet to resonance. We employ a spin-torque ferromagnetic resonance excitation/detection scheme which was developed originally for a bulk spin-orbital effect, the spin Hall effect. In our experiment, the direct Rashba-Edelstein effect generates an oscillating spin current from an alternating charge current driving the magnetization precession in a neighboring permalloy (Py, Ni80Fe20) layer. Electrical detection of the magnetization dynamics is achieved by a rectificationmechanism of the time dependent multilayer resistance arising from the anisotropic magnetoresistance. C1 [Jungfleisch, M. B.; Zhang, W.; Sklenar, J.; Jiang, W.; Pearson, J. E.; Hoffmann, A.] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. [Sklenar, J.; Ketterson, J. B.] Northwestern Univ, Dept Phys & Astron, Evanston, IL 60208 USA. RP Jungfleisch, MB (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM jungfleisch@anl.gov RI Jungfleisch, Matthias Benjamin/G-1069-2015 OI Jungfleisch, Matthias Benjamin/0000-0001-8204-3677 FU U.S. Department of Energy, Office of Science, Materials Science and Engineering Division; DOE, Office of Science, Basic Energy Science [DE-AC02-06CH11357] FX We thank Roland Winkler for illuminating discussions. This work was supported by the U.S. Department of Energy, Office of Science, Materials Science and Engineering Division. Lithography was carried out at the Center for Nanoscale Materials, an Office of Science user facility, which is supported by DOE, Office of Science, Basic Energy Science under Contract No. DE-AC02-06CH11357. NR 39 TC 2 Z9 2 U1 13 U2 24 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUN 20 PY 2016 VL 93 IS 22 AR 224419 DI 10.1103/PhysRevB.93.224419 PG 5 WC Physics, Condensed Matter SC Physics GA DO9KD UT WOS:000378104200009 ER PT J AU Martin, I Gopalakrishnan, S Demler, EA AF Martin, Ivar Gopalakrishnan, Sarang Demler, Eugene A. TI Weak crystallization theory of metallic alloys SO PHYSICAL REVIEW B LA English DT Article ID DENSITY-FUNCTIONAL THEORY; MEAN-FIELD-THEORY; QUASI-CRYSTALS; ORIENTATIONAL ORDER; PATTERN SELECTION; FARADAY WAVES; PHASE; QUASICRYSTALS; GLASSES AB Crystallization is one of the most familiar, but hardest to analyze, phase transitions. The principal reason is that crystallization typically occurs via a strongly first-order phase transition, and thus rigorous treatment would require comparing energies of an infinite number of possible crystalline states with the energy of liquid. A great simplification occurs when crystallization transition happens to be weakly first order. In this case, weak crystallization theory, based on unbiased Ginzburg-Landau expansion, can be applied. Even beyond its strict range of validity, it has been a useful qualitative tool for understanding crystallization. In its standard form, however, weak crystallization theory cannot explain the existence of a majority of observed crystalline and quasicrystalline states. Here we extend the weak crystallization theory to the case of metallic alloys. We identify a singular effect of itinerant electrons on the form of weak crystallization free energy. It is geometric in nature, generating strong dependence of free energy on the angles between ordering wave vectors of ionic density. That leads to stabilization of fcc, rhombohedral, and icosahedral quasicrystalline (iQC) phases, which are absent in the generic theory with only local interactions. As an application, we find the condition for stability of iQC that is consistent with the Hume-Rothery rules known empirically for the majority of stable iQC; namely, the length of the primary Bragg-peak wave vector is approximately equal to the diameter of the Fermi sphere. C1 [Martin, Ivar] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. [Gopalakrishnan, Sarang; Demler, Eugene A.] Harvard Univ, Dept Phys, Cambridge, MA 02138 USA. [Gopalakrishnan, Sarang] CALTECH, Dept Phys, Pasadena, CA 91125 USA. RP Martin, I (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. FU Department of Energy, Office of Basic Energy Science, Materials Science and Engineering Division; Harvard-MIT CUA; NSF Grant [DMR-1308435]; AFOSR Quantum Simulation MURI; Walter Burke Institute at Caltech; Humboldt Foundation FX Authors would like to thank P. Goldbart, Z. Nussinov, D. Levine, P. Steinhardt, J. Vinals, and A. Rosch for useful discussions. I.M. acknowledges support from Department of Energy, Office of Basic Energy Science, Materials Science and Engineering Division. S.G. and E.A.D. acknowledge support from Harvard-MIT CUA, NSF Grant No. DMR-1308435, and AFOSR Quantum Simulation MURI. S.G. acknowledges support from the Walter Burke Institute at Caltech. E.A.D. acknowledges support from the Humboldt Foundation. NR 37 TC 1 Z9 1 U1 1 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUN 20 PY 2016 VL 93 IS 23 AR 235140 DI 10.1103/PhysRevB.93.235140 PG 9 WC Physics, Condensed Matter SC Physics GA DO9KO UT WOS:000378105400007 ER PT J AU McClain, J Lischner, J Watson, T Matthews, DA Ronca, E Louie, SG Berkelbach, TC Chan, GKL AF McClain, James Lischner, Johannes Watson, Thomas Matthews, Devin A. Ronca, Enrico Louie, Steven G. Berkelbach, Timothy C. Chan, Garnet Kin-Lic TI Spectral functions of the uniform electron gas via coupled-cluster theory and comparison to the GW and related approximations SO PHYSICAL REVIEW B LA English DT Article ID SINGLE-PARTICLE SPECTRUM; SELF-CONSISTENT GW; T-MATRIX THEORY; GREENS-FUNCTION; CUMULANT EXPANSION; BAND-STRUCTURE; METALS; NA; ENERGIES; SYSTEMS AB We use ab initio coupled-cluster theory to compute the spectral function of the uniform electron gas at a Wigner-Seitz radius of r(s) = 4. The coupled-cluster approximations we employ go significantly beyond the diagrammatic content of state-of-the-art GW theory. We compare our calculations extensively to GW and GW-plus-cumulant theory, illustrating the strengths and weaknesses of these methods in capturing the quasiparticle and satellite features of the electron gas. Our accurate calculations further allow us to address the long-standing debate over the occupied bandwidth of metallic sodium. Our findings indicate that the future application of coupled-cluster theory to condensed phase material spectra is highly promising. C1 [McClain, James; Watson, Thomas; Ronca, Enrico; Chan, Garnet Kin-Lic] Princeton Univ, Dept Chem, Princeton, NJ 08544 USA. [Lischner, Johannes] Univ London Imperial Coll Sci Technol & Med, Dept Phys, London SW7 2AZ, England. [Lischner, Johannes] Univ London Imperial Coll Sci Technol & Med, Dept Mat, London SW7 2AZ, England. [Lischner, Johannes] Univ London Imperial Coll Sci Technol & Med, Thomas Young Ctr Theory & Simulat Mat, London SW7 2AZ, England. [Lischner, Johannes; Louie, Steven G.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Lischner, Johannes; Louie, Steven G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Matthews, Devin A.] Univ Texas Austin, Inst Computat Engn & Sci, Austin, TX 78712 USA. [Berkelbach, Timothy C.; Chan, Garnet Kin-Lic] Princeton Univ, Princeton Ctr Theoret Sci, Princeton, NJ 08544 USA. RP McClain, J (reprint author), Princeton Univ, Dept Chem, Princeton, NJ 08544 USA. FU Engineering and Physical Sciences Research Council [EP/N005244/1]; Thomas Young Centre [TYC-101]; SciDAC Program on Excited State Phenomena in Energy Materials - U.S. Department of Energy (DOE); Office of Basic Energy Sciences and of Advanced Scientific Computing Research [DE-AC02-05CH11231]; NSF [DMR15-1508412]; National Science Foundation [ACI-1148125]; Computational Laboratory for Hybrid/Organic Photovoltaics of CNR-ISTM for a fellowship - CNR-EFOR project; Princeton Center for Theoretical Science; DOE (SciDAC): Predictive Computing for Condensed Matter [DE-SC0008624]; DOE: Quantum Embedding for Correlated Electronic Structure in Large Systems; Condensed Phase [DE-SC0010530]; Simons Foundation through the Simons Collaboration FX CCSD calculations were carried out using a modified version of the ACES III code [61] through the University of Florida High Performance Computing Center. CCSDT calculations were performed using a modified version of the CFOUR code [62]. Dynamical density-matrix renormalization-group calculations were done with the BLOCK code [63-65]. J.L. acknowledges support from Engineering and Physical Sciences Research Council under Grant No. EP/N005244/1 and also from the Thomas Young Centre under Grant No. TYC-101. S.G.L. and J.L. acknowledge support by the SciDAC Program on Excited State Phenomena in Energy Materials funded by the U.S. Department of Energy (DOE), Office of Basic Energy Sciences and of Advanced Scientific Computing Research, under Contract No. DE-AC02-05CH11231 at Lawrence Berkeley National Laboratory (algorithm and code development) and by the NSF under Grant No. DMR15-1508412 (basic theory and formalism). D.A.M. is supported at the University of Texas by the National Science Foundation (Grant No. ACI-1148125). E.R. acknowledges the Computational Laboratory for Hybrid/Organic Photovoltaics of CNR-ISTM for a fellowship funded by the CNR-EFOR project. T.C.B. is supported by the Princeton Center for Theoretical Science. J.M., T.W., E.R., and G.K.-L.C. acknowledge primary support from DOE (SciDAC): Predictive Computing for Condensed Matter under Contract No. DE-SC0008624, and additional funding from DOE: Quantum Embedding for Correlated Electronic Structure in Large Systems and the Condensed Phase under Contract No. DE-SC0010530. G.K.-L.C. also acknowledges support from the Simons Foundation through the Simons Collaboration on the Many Electron Problem. NR 64 TC 5 Z9 5 U1 3 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUN 20 PY 2016 VL 93 IS 23 AR 235139 DI 10.1103/PhysRevB.93.235139 PG 6 WC Physics, Condensed Matter SC Physics GA DO9KO UT WOS:000378105400006 ER PT J AU Qiu, DY da Jornada, FH Louie, SG AF Qiu, Diana Y. da Jornada, Felipe H. Louie, Steven G. TI Screening and many-body effects in two-dimensional crystals: Monolayer MoS2 SO PHYSICAL REVIEW B LA English DT Article ID ELECTRON-HOLE EXCITATIONS; QUASI-PARTICLE ENERGIES; MOLYBDENUM-DISULFIDE; OPTICAL-SPECTRA; SEMICONDUCTORS; STATES; INSULATORS; BANDGAP; PHOTOLUMINESCENCE; SPECTROSCOPY AB We present a systematic study of the variables affecting the electronic and optical properties of two-dimensional (2D) crystals within ab initio GW and GW plus Bethe-Salpeter equation (GW-BSE) calculations. As a prototypical 2D transition metal dichalcogenide material, we focus our study on monolayer MoS2. We find that the reported variations in GW-BSE results in the literature for monolayer MoS2 and related systems arise from different treatments of the long-range Coulomb interaction in supercell calculations and convergence of k-grid sampling and cutoffs for various quantities such as the dielectric screening. In particular, the quasi-2D nature of the system gives rise to fast spatial variations in the screening environment, which are computationally challenging to resolve. We also show that common numerical treatments to remove the divergence in the Coulomb interaction can shift the exciton continuum leading to false convergence with respect to k-point sampling. Our findings apply to GW-BSE calculations on any low-dimensional semiconductors. C1 [Louie, Steven G.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Louie, SG (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM sglouie@berkeley.edu FU Office of Basic Energy Sciences, U.S. Department of Energy [DE-AC02-05CH11231]; NSF [DMR15-1508412]; NSF Graduate Research Fellowship [DGE 1106400]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; National Science Foundation [787 ACI-1053575] FX We thank L. Yang and T. Cao for discussions. This research was supported by the Theory Program (which provided the GW-BSE calculations) and by the SciDAC Program on Excited State Phenomena (which provided methods and software developments) at the Lawrence Berkeley National Lab through the Office of Basic Energy Sciences, U.S. Department of Energy under Contract No. DE-AC02-05CH11231, and by NSF Grant No. DMR15-1508412 (which provided structural study and electron-phonon interaction effects on the optical spectra). D.Y.Q. acknowledges support from the NSF Graduate Research Fellowship Grant No. DGE 1106400. This research used resources of the National Energy Research Scientific Computing Center (NERSC), a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231, and the Extreme Science and Engineering Discovery Environment (XSEDE), which is supported by National Science Foundation Grant No. 787 ACI-1053575. NR 56 TC 5 Z9 5 U1 22 U2 51 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUN 20 PY 2016 VL 93 IS 23 AR 235435 DI 10.1103/PhysRevB.93.235435 PG 12 WC Physics, Condensed Matter SC Physics GA DO9KO UT WOS:000378105400014 ER PT J AU van Roekeghem, A Richard, P Shi, X Wu, SF Zeng, LK Saparov, B Ohtsubo, Y Qian, T Sefat, AS Biermann, S Ding, H AF van Roekeghem, Ambroise Richard, Pierre Shi, Xun Wu, Shangfei Zeng, Lingkun Saparov, Bayrammurad Ohtsubo, Yoshiyuki Qian, Tian Sefat, Athena S. Biermann, Silke Ding, Hong TI Tetragonal and collapsed-tetragonal phases of CaFe2As2: A view from angle-resolved photoemission and dynamical mean-field theory SO PHYSICAL REVIEW B LA English DT Article ID CORRELATED SYSTEMS; SRVO3 AB We present a study of the tetragonal to collapsed-tetragonal transition of CaFe2As2 using angle-resolved photoemission spectroscopy and dynamical mean field theory-based electronic structure calculations. We observe that the collapsed-tetragonal phase exhibits reduced correlations and a higher coherence temperature due to the stronger Fe-As hybridization. Furthermore, a comparison of measured photoemission spectra and theoretical spectral functions shows that momentum-dependent corrections to the density functional band structure are essential for the description of low-energy quasiparticle dispersions. We introduce those using the recently proposed combined "screened exchange + dynamical mean field theory" scheme. C1 [van Roekeghem, Ambroise; Richard, Pierre; Shi, Xun; Wu, Shangfei; Zeng, Lingkun; Qian, Tian; Ding, Hong] Chinese Acad Sci, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China. [van Roekeghem, Ambroise; Richard, Pierre; Shi, Xun; Wu, Shangfei; Zeng, Lingkun; Qian, Tian; Ding, Hong] Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China. [van Roekeghem, Ambroise; Biermann, Silke] Univ Paris Saclay, CNRS, Ecole Polytech, Ctr Phys Theor, F-91128 Palaiseau, France. [Richard, Pierre; Ding, Hong] Collaborat Innovat Ctr Quantum Matter, Beijing, Peoples R China. [Shi, Xun] Paul Scherrer Inst, Swiss Light Source, CH-5232 Villigen, Switzerland. [Saparov, Bayrammurad; Sefat, Athena S.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Ohtsubo, Yoshiyuki] Synchrotron SOLEIL, St Aubin BP 48, F-91192 Gif Sur Yvette, France. [Biermann, Silke] Coll France, 11 Pl Marcelin Berthelot, F-75005 Paris, France. [Biermann, Silke] European Theoret Synchrotron Facil, Grenoble, France. RP van Roekeghem, A (reprint author), Chinese Acad Sci, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China.; van Roekeghem, A (reprint author), Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China.; van Roekeghem, A (reprint author), Univ Paris Saclay, CNRS, Ecole Polytech, Ctr Phys Theor, F-91128 Palaiseau, France. EM vanroeke@cpht.polytechnique.fr RI Richard, Pierre/F-7652-2010; Ohtsubo, Yoshiyuki/O-2052-2016; Sefat, Athena/R-5457-2016; Biermann, Silke/D-5603-2013 OI Richard, Pierre/0000-0003-0544-4551; Ohtsubo, Yoshiyuki/0000-0003-4388-825X; Sefat, Athena/0000-0002-5596-3504; Biermann, Silke/0000-0002-3884-0385 FU Cai Yuanpei program, IDRIS/GENCI Orsay [t2015091393]; European Research Council [617196]; NSF from China [NSF PHY11-25915]; MOST from China [2010CB923000, 2011CBA001000, 2011CBA00102, 2012CB821403]; NSFC from China [10974175, 11004232, 11034011/A0402, 11234014, 11274362]; US Department of Energy, Office of Science, Basic Energy Sciences, Materials Science, and Engineering Division FX We acknowledge useful discussions with Veronique Brouet and we are grateful to Thomas Ayral, Michel Ferrero, and Olivier Parcollet for support on the TRIQS toolkit [37]. We acknowledge SOLEIL for provision of synchrotron radiation facilities and we would like to thank Franccois Bertran, Patrick Le Fevre, and Amina Taleb for assistance in using the beamline CASSIOPEE. This work was supported by the Cai Yuanpei program, IDRIS/GENCI Orsay under Project No. t2015091393, the European Research Council under Project No. 617196, the NSF under Grant No. NSF PHY11-25915, MOST (Grants No. 2010CB923000, No. 2011CBA001000, No. 2011CBA00102, and No. 2012CB821403) and NSFC (Grants No. 10974175, No. 11004232, No. 11034011/A0402, No. 11234014, and No. 11274362) from China. The work at Oak Ridge National Laboratory was primarily supported by the US Department of Energy, Office of Science, Basic Energy Sciences, Materials Science, and Engineering Division. NR 37 TC 2 Z9 2 U1 5 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUN 20 PY 2016 VL 93 IS 24 AR 245139 DI 10.1103/PhysRevB.93.245139 PG 9 WC Physics, Condensed Matter SC Physics GA DO9KX UT WOS:000378106400004 ER PT J AU Huang, Y Zhu, SJ Hamilton, JH Wang, EH Ramayya, AV Xiao, ZG Li, HJ Luo, YX Rasmussen, JO Ter-Akopian, GM Oganessian, YT AF Huang, Y. Zhu, S. J. Hamilton, J. H. Wang, E. H. Ramayya, A. V. Xiao, Z. G. Li, H. J. Luo, Y. X. Rasmussen, J. O. Ter-Akopian, G. M. Oganessian, Yu. Ts. TI Proposed s = +/- 1 octupole bands in Xe-140 SO PHYSICAL REVIEW C LA English DT Article ID RICH XE ISOTOPES; HIGH-SPIN STATES; NEUTRON-RICH; SPONTANEOUS FISSION; BARIUM ISOTOPES; NUCLEI; DEFORMATION; PARITY; TH-222; ARRAYS AB Level structures of neutron-rich Xe-140 nucleus have been reinvestigated by using a triple gamma coincidence study from the spontaneous fission of Cf-252. Several new levels and transitions are identified. The previously observed s = +1 octupole band structure is confirmed and expanded. Another set of the Delta I = 2 positive and negative parity bands connected by strong E1 transitions is proposed as the s = -1 octupole band structure. Thus, the s = +/- 1 doublet octupole bands are completed in Xe-140. The experimental B(E1)/B(E2) branching ratios indicate that the octupole correlations in Xe-140 are weak. The other characteristics of the s = +/- 1 octupole bands have been discussed. C1 [Huang, Y.; Zhu, S. J.; Xiao, Z. G.; Li, H. J.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Hamilton, J. H.; Wang, E. H.; Ramayya, A. V.; Luo, Y. X.] Vanderbilt Univ, Dept Phys, Nashville, TN 37235 USA. [Luo, Y. X.; Rasmussen, J. O.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Ter-Akopian, G. M.; Oganessian, Yu. Ts.] Joint Inst Nucl Res, RU-141980 Dubna, Russia. RP Zhu, SJ (reprint author), Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. EM zhushj@mail.tsinghua.edu.cn FU National Natural Science Foundation of China [11175095, 11205112, 11375094]; Tsinghua University Initiative Scientific Research Program; U.S. Department of Energy [DE-FG05-88ER40407, DE-AC03-76SF00098] FX The work at Tsinghua University was supported by the National Natural Science Foundation of China under Grants No. 11175095, No. 11205112, and No. 11375094, and by Tsinghua University Initiative Scientific Research Program. The work at Vanderbilt University, Lawrence Berkeley National Laboratory was supported by THE U.S. Department of Energy under Grant No. DE-FG05-88ER40407 and Contract No. DE-AC03-76SF00098. NR 39 TC 0 Z9 0 U1 5 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD JUN 20 PY 2016 VL 93 IS 6 AR 064321 DI 10.1103/PhysRevC.93.064321 PG 9 WC Physics, Nuclear SC Physics GA DO9LX UT WOS:000378109200003 ER PT J AU Perez-Loureiro, D Wrede, C Bennett, MB Liddick, SN Bowe, A Brown, BA Chen, AA Chipps, KA Cooper, N Irvine, D McNeice, E Montes, F Naqvi, F Ortez, R Pain, SD Pereira, J Prokop, CJ Quaglia, J Quinn, SJ Sakstrup, J Santia, M Schwartz, SB Shanab, S Simon, A Spyrou, A Thiagalingam, E AF Perez-Loureiro, D. Wrede, C. Bennett, M. B. Liddick, S. N. Bowe, A. Brown, B. A. Chen, A. A. Chipps, K. A. Cooper, N. Irvine, D. McNeice, E. Montes, F. Naqvi, F. Ortez, R. Pain, S. D. Pereira, J. Prokop, C. J. Quaglia, J. Quinn, S. J. Sakstrup, J. Santia, M. Schwartz, S. B. Shanab, S. Simon, A. Spyrou, A. Thiagalingam, E. TI beta-delayed gamma decay of P-26: Possible evidence of a proton halo SO PHYSICAL REVIEW C LA English DT Article ID INTERACTION CROSS-SECTIONS; VECTOR COUPLING-CONSTANT; SD-SHELL NUCLEI; 2ND-CLASS CURRENTS; MIRROR NUCLEI; 2-PROTON HALO; LIGHT-NUCLEI; C-9; SPECTROSCOPY; RATES AB Background: Measurements of beta decay provide important nuclear structure information that can be used to probe isospin asymmetries and inform nuclear astrophysics studies. Purpose: To measure the beta-delayed gamma decay of P-26 and compare the results with previous experimental results and shell-model calculations. Method: A P-26 fast beam produced using nuclear fragmentation was implanted into a planar germanium detector. Its beta-delayed gamma-ray emission was measured with an array of 16 high-purity germanium detectors. Positrons emitted in the decay were detected in coincidence to reduce the background. Results: The absolute intensities of P-26 beta-delayed gamma rays were determined. A total of six new beta-decay branches and 15 new gamma-ray lines have been observed for the first time in P-26 beta decay. A complete beta-decay scheme was built for the allowed transitions to bound excited states of Si-26. f t values and Gamow-Teller strengths were also determined for these transitions and compared with shell-model calculations and the mirror beta decay of Na-26, revealing significant mirror asymmetries. Conclusions: A very good agreement with theoretical predictions based on the USDB shell model is observed. The significant mirror asymmetry observed for the transition to the first excited state (delta = 51(10)%) may be evidence for a proton halo in P-26. C1 [Perez-Loureiro, D.; Wrede, C.; Bennett, M. B.; Liddick, S. N.; Bowe, A.; Brown, B. A.; Montes, F.; Ortez, R.; Pereira, J.; Prokop, C. J.; Quaglia, J.; Quinn, S. J.; Sakstrup, J.; Santia, M.; Schwartz, S. B.; Shanab, S.; Simon, A.; Spyrou, A.] Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA. [Wrede, C.; Bennett, M. B.; Bowe, A.; Brown, B. A.; Ortez, R.; Quinn, S. J.; Sakstrup, J.; Santia, M.; Schwartz, S. B.; Shanab, S.; Spyrou, A.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Liddick, S. N.; Prokop, C. J.] Michigan State Univ, Dept Chem, E Lansing, MI 48824 USA. [Bowe, A.] Kalamazoo Coll, Dept Phys, Kalamazoo, MI 49006 USA. [Chen, A. A.; Irvine, D.; McNeice, E.; Thiagalingam, E.] McMaster Univ, Dept Phys & Astron, Hamilton, ON L8S 4M1, Canada. [Chipps, K. A.] Colorado Sch Mines, Dept Phys, Golden, CO 80401 USA. [Chipps, K. A.; Pain, S. D.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Chipps, K. A.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Cooper, N.; Naqvi, F.] Yale Univ, Dept Phys, New Haven, CT 06520 USA. [Cooper, N.; Naqvi, F.] Yale Univ, Wright Nucl Struct Lab, New Haven, CT 06520 USA. [Pereira, J.; Quaglia, J.; Quinn, S. J.; Spyrou, A.] Michigan State Univ, Joint Inst Nucl Astrophys, E Lansing, MI 48824 USA. [Ortez, R.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Quaglia, J.] Michigan State Univ, Dept Elect Engn, E Lansing, MI 48824 USA. [Schwartz, S. B.] Univ So Indiana, Geol & Phys Dept, Evansville, IN 47712 USA. [Simon, A.] Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. [Simon, A.] Univ Notre Dame, Joint Inst Nucl Astrophys, Notre Dame, IN 46556 USA. RP Perez-Loureiro, D (reprint author), Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA. EM perezlou@nscl.msu.edu; wrede@nscl.msu.edu OI Perez-Loureiro, David/0000-0002-0609-1308 FU U.S. National Science Foundation [PHY-1102511, PHY-0822648, PHY-1350234, PHY-1404442]; U.S. Department of Energy [DE-FG02-97ER41020]; U.S. National Nuclear Security Agency [DE-NA0000979]; Natural Sciences and Engineering Research Council of Canada FX The authors gratefully acknowledge the contributions of the NSCL staff. This work is supported by the U.S. National Science Foundation under Grants No. PHY-1102511, No. PHY-0822648, No. PHY-1350234, and No. PHY-1404442, the U.S. Department of Energy under Contract No. DE-FG02-97ER41020, the U.S. National Nuclear Security Agency under Contract No. DE-NA0000979, and the Natural Sciences and Engineering Research Council of Canada. NR 57 TC 1 Z9 1 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD JUN 20 PY 2016 VL 93 IS 6 AR 064320 DI 10.1103/PhysRevC.93.064320 PG 15 WC Physics, Nuclear SC Physics GA DO9LX UT WOS:000378109200002 ER PT J AU Aaltonen, T Amerio, S Amidei, D Anastassov, A Annovi, A Antos, J Apollinari, G Appel, JA Arisawa, T Artikov, A Asaadi, J Ashmanskas, W Auerbach, B Aurisano, A Azfar, F Badgett, W Bae, T Barbaro-Galtieri, A Barnes, VE Barnett, BA Barria, P Bartos, P Bauce, M Bedeschi, F Behari, S Bellettini, G Bellinger, J Benjamin, D Beretvas, A Bhatti, A Bland, KR Blumenfeld, B Bocci, A Bodek, A Bortoletto, D Boudreau, J Boveia, A Brigliadori, L Bromberg, C Brucken, E Budagov, J Budd, HS Burkett, K Busetto, G Bussey, P Butti, P Buzatu, A Calamba, A Camarda, S Campanelli, M Canelli, F Carls, B Carlsmith, D Carosi, R Carrillo, S Casal, B Casarsa, M Castro, A Catastini, P Cauz, D Cavaliere, V Cerri, A Cerrito, L Chen, YC Chertok, M Chiarelli, G Chlachidze, G Cho, K Chokheli, D Clark, A Clarke, C Convery, ME Conway, J Corbo, M Cordelli, M Cox, CA Cox, DJ Cremonesi, M Cruz, D Cuevas, J Culbertson, R d'Ascenzo, N Datta, M de Barbaro, P Demortier, L Deninno, M D'Errico, M Devoto, F Di Canto, A Di Ruzza, B Dittmann, JR Donati, S D'Onofrio, M Dorigo, M Driutti, A Ebina, K Edgar, R Erbacher, R Errede, S Esham, B Farrington, S Ramos, JPF Field, R Flanagan, G Forrest, R Franklin, M Freeman, JC Frisch, H Funakoshi, Y Galloni, C Garfinkel, AF Garosi, P Gerberich, H Gerchtein, E Giagu, S Giakoumopoulou, V Gibson, K Ginsburg, CM Giokaris, N Giromini, P Glagolev, V Glenzinski, D Gold, M Goldin, D Golossanov, A Gomez, G Gomez-Ceballos, G Goncharov, M Lopez, OG Gorelov, I Goshaw, AT Goulianos, K Gramellini, E Grosso-Pilcher, C da Costa, JG Hahn, SR Han, JY Happacher, F Hara, K Hare, M Harr, RF Harrington-Taber, T Hatakeyama, K Hays, C Heinrich, J Herndon, M Hocker, A Hong, Z Hopkins, W Hou, S Hughes, RE Husemann, U Hussein, M Huston, J Introzzi, G Iori, M Ivanov, A James, E Jang, D Jayatilaka, B Jeon, EJ Jindariani, S Jones, M Joo, KK Jun, SY Junk, TR Kambeitz, M Kamon, T Karchin, PE Kasmi, A Kato, Y Ketchum, W Keung, J Kilminster, B Kim, DH Kim, HS Kim, JE Kim, MJ Kim, SH Kim, SB Kim, YJ Kim, YK Kimura, N Kirby, M Knoepfel, K Kondo, K Kong, DJ Konigsberg, J Kotwal, AV Kreps, M Kroll, J Kruse, M Kuhr, T Kurata, M Laasanen, AT Lammel, S Lancaster, M Lannon, K Latino, G Lee, HS Lee, JS Leo, S Leone, S Lewis, JD Limosani, A Lipeles, E Lister, A Liu, Q Liu, T Lockwitz, S Loginov, A Lucchesi, D Luca, A Lueck, J Lujan, P Lukens, P Lungu, G Lys, J Lysak, R Madrak, R Maestro, P Malik, S Manca, G Manousakis-Katsikakis, A Marchese, L Margaroli, F Marino, P Matera, K Mattson, ME Mazzacane, A Mazzanti, P McNulty, R Mehta, A Mehtala, P Mesropian, C Miao, T Mietlicki, D Mitra, A Miyake, H Moed, S Moggi, N Moon, CS Moore, R Morello, MJ Mukherjee, A Muller, T Murat, P Mussini, M Nachtman, J Nagai, Y Naganoma, J Nakano, I Napier, A Nett, J Nigmanov, T Nodulman, L Noh, SY Norniella, O Oakes, L Oh, SH Oh, YD Okusawa, T Orava, R Ortolan, L Pagliarone, C Palencia, E Palni, P Papadimitriou, V Parker, W Pauletta, G Paulini, M Paus, C Phillips, TJ Piacentino, G Pianori, E Pilot, J Pitts, K Plager, C Pondrom, L Poprocki, S Potamianos, K Pranko, A Prokoshin, F Ptohos, F Punzi, G Fernandez, IR Renton, P Rescigno, M Rimondi, F Ristori, L Robson, A Rodriguez, T Rolli, S Ronzani, M Roser, R Rosner, JL Ruffini, F Ruiz, A Russ, J Rusu, V Sakumoto, WK Sakurai, Y Santi, L Sato, K Saveliev, V Savoy-Navarro, A Schlabach, P Schmidt, EE Schwarz, T Scodellaro, L Scuri, F Seidel, S Seiya, Y Semenov, A Sforza, F Shalhout, SZ Shears, T Shepard, PF Shimojima, M Shochet, M Shreyber-Tecker, I Simonenko, A Sliwa, K Smith, JR Snider, FD Song, H Sorin, V Denis, RS Stancari, M Stentz, D Strologas, J Sudo, Y Sukhanov, A Suslov, I Takemasa, K Takeuchi, Y Tang, J Tecchio, M Teng, PK Thom, J Thomson, E Thukral, V Toback, D Tokar, S Tollefson, K Tomura, T Tonelli, D Torre, S Torretta, D Totaro, P Trovato, M Ukegawa, F Uozumi, S Vazquez, F Velev, G Vellidis, C Vernieri, C Vidal, M Vilar, R Vizan, J Vogel, M Volpi, G Wagner, P Wallny, R Wang, SM Waters, D Wester, WC Whiteson, D Wicklund, AB Wilbur, S Williams, HH Wilson, JS Wilson, P Winer, BL Wittich, P Wolbers, S Wolfe, H Wright, T Wu, X Wu, Z Yamamoto, K Yamato, D Yang, T Yang, UK Yang, YC Yao, WM Yeh, GP Yi, K Yoh, J Yorita, K Yoshida, T Yu, GB Yu, I Zanetti, AM Zeng, Y Zhou, C Zucchelli, S AF Aaltonen, T. Amerio, S. Amidei, D. Anastassov, A. Annovi, A. Antos, J. Apollinari, G. Appel, J. A. Arisawa, T. Artikov, A. Asaadi, J. Ashmanskas, W. Auerbach, B. Aurisano, A. Azfar, F. Badgett, W. Bae, T. Barbaro-Galtieri, A. Barnes, V. E. Barnett, B. A. Barria, P. Bartos, P. Bauce, M. Bedeschi, F. Behari, S. Bellettini, G. Bellinger, J. Benjamin, D. Beretvas, A. Bhatti, A. Bland, K. R. Blumenfeld, B. Bocci, A. Bodek, A. Bortoletto, D. Boudreau, J. Boveia, A. Brigliadori, L. Bromberg, C. Brucken, E. Budagov, J. Budd, H. S. Burkett, K. Busetto, G. Bussey, P. Butti, P. Buzatu, A. Calamba, A. Camarda, S. Campanelli, M. Canelli, F. Carls, B. Carlsmith, D. Carosi, R. Carrillo, S. Casal, B. Casarsa, M. Castro, A. Catastini, P. Cauz, D. Cavaliere, V. Cerri, A. Cerrito, L. Chen, Y. C. Chertok, M. Chiarelli, G. Chlachidze, G. Cho, K. Chokheli, D. Clark, A. Clarke, C. Convery, M. E. Conway, J. Corbo, M. Cordelli, M. Cox, C. A. Cox, D. J. Cremonesi, M. Cruz, D. Cuevas, J. Culbertson, R. d'Ascenzo, N. Datta, M. de Barbaro, P. Demortier, L. Deninno, M. D'Errico, M. Devoto, F. Di Canto, A. Di Ruzza, B. Dittmann, J. R. Donati, S. D'Onofrio, M. Dorigo, M. Driutti, A. Ebina, K. Edgar, R. Erbacher, R. Errede, S. Esham, B. Farrington, S. Fernandez Ramos, J. P. Field, R. Flanagan, G. Forrest, R. Franklin, M. Freeman, J. C. Frisch, H. Funakoshi, Y. Galloni, C. Garfinkel, A. F. Garosi, P. Gerberich, H. Gerchtein, E. Giagu, S. Giakoumopoulou, V. Gibson, K. Ginsburg, C. M. Giokaris, N. Giromini, P. Glagolev, V. Glenzinski, D. Gold, M. Goldin, D. Golossanov, A. Gomez, G. Gomez-Ceballos, G. Goncharov, M. Gonzalez Lopez, O. Gorelov, I. Goshaw, A. T. Goulianos, K. Gramellini, E. Grosso-Pilcher, C. da Costa, J. Guimaraes Hahn, S. R. Han, J. Y. Happacher, F. Hara, K. Hare, M. Harr, R. F. Harrington-Taber, T. Hatakeyama, K. Hays, C. Heinrich, J. Herndon, M. Hocker, A. Hong, Z. Hopkins, W. Hou, S. Hughes, R. E. Husemann, U. Hussein, M. Huston, J. Introzzi, G. Iori, M. Ivanov, A. James, E. Jang, D. Jayatilaka, B. Jeon, E. J. Jindariani, S. Jones, M. Joo, K. K. Jun, S. Y. Junk, T. R. Kambeitz, M. Kamon, T. Karchin, P. E. Kasmi, A. Kato, Y. Ketchum, W. Keung, J. Kilminster, B. Kim, D. H. Kim, H. S. Kim, J. E. Kim, M. J. Kim, S. H. Kim, S. B. Kim, Y. J. Kim, Y. K. Kimura, N. Kirby, M. Knoepfel, K. Kondo, K. Kong, D. J. Konigsberg, J. Kotwal, A. V. Kreps, M. Kroll, J. Kruse, M. Kuhr, T. Kurata, M. Laasanen, A. T. Lammel, S. Lancaster, M. Lannon, K. Latino, G. Lee, H. S. Lee, J. S. Leo, S. Leone, S. Lewis, J. D. Limosani, A. Lipeles, E. Lister, A. Liu, Q. Liu, T. Lockwitz, S. Loginov, A. Lucchesi, D. Luca, A. Lueck, J. Lujan, P. Lukens, P. Lungu, G. Lys, J. Lysak, R. Madrak, R. Maestro, P. Malik, S. Manca, G. Manousakis-Katsikakis, A. Marchese, L. Margaroli, F. Marino, P. Matera, K. Mattson, M. E. Mazzacane, A. Mazzanti, P. McNulty, R. Mehta, A. Mehtala, P. Mesropian, C. Miao, T. Mietlicki, D. Mitra, A. Miyake, H. Moed, S. Moggi, N. Moon, C. S. Moore, R. Morello, M. J. Mukherjee, A. Muller, Th. Murat, P. Mussini, M. Nachtman, J. Nagai, Y. Naganoma, J. Nakano, I. Napier, A. Nett, J. Nigmanov, T. Nodulman, L. Noh, S. Y. Norniella, O. Oakes, L. Oh, S. H. Oh, Y. D. Okusawa, T. Orava, R. Ortolan, L. Pagliarone, C. Palencia, E. Palni, P. Papadimitriou, V. Parker, W. Pauletta, G. Paulini, M. Paus, C. Phillips, T. J. Piacentino, G. Pianori, E. Pilot, J. Pitts, K. Plager, C. Pondrom, L. Poprocki, S. Potamianos, K. Pranko, A. Prokoshin, F. Ptohos, F. Punzi, G. Redondo Fernandez, I. Renton, P. Rescigno, M. Rimondi, F. Ristori, L. Robson, A. Rodriguez, T. Rolli, S. Ronzani, M. Roser, R. Rosner, J. L. Ruffini, F. Ruiz, A. Russ, J. Rusu, V. Sakumoto, W. K. Sakurai, Y. Santi, L. Sato, K. Saveliev, V. Savoy-Navarro, A. Schlabach, P. Schmidt, E. E. Schwarz, T. Scodellaro, L. Scuri, F. Seidel, S. Seiya, Y. Semenov, A. Sforza, F. Shalhout, S. Z. Shears, T. Shepard, P. F. Shimojima, M. Shochet, M. Shreyber-Tecker, I. Simonenko, A. Sliwa, K. Smith, J. R. Snider, F. D. Song, H. Sorin, V. Denis, R. St. Stancari, M. Stentz, D. Strologas, J. Sudo, Y. Sukhanov, A. Suslov, I. Takemasa, K. Takeuchi, Y. Tang, J. Tecchio, M. Teng, P. K. Thom, J. Thomson, E. Thukral, V. Toback, D. Tokar, S. Tollefson, K. Tomura, T. Tonelli, D. Torre, S. Torretta, D. Totaro, P. Trovato, M. Ukegawa, F. Uozumi, S. Vazquez, F. Velev, G. Vellidis, C. Vernieri, C. Vidal, M. Vilar, R. Vizan, J. Vogel, M. Volpi, G. Wagner, P. Wallny, R. Wang, S. M. Waters, D. Wester, W. C., III Whiteson, D. Wicklund, A. B. Wilbur, S. Williams, H. H. Wilson, J. S. Wilson, P. Winer, B. L. Wittich, P. Wolbers, S. Wolfe, H. Wright, T. Wu, X. Wu, Z. Yamamoto, K. Yamato, D. Yang, T. Yang, U. K. Yang, Y. C. Yao, W. -M. Yeh, G. P. Yi, K. Yoh, J. Yorita, K. Yoshida, T. Yu, G. B. Yu, I. Zanetti, A. M. Zeng, Y. Zhou, C. Zucchelli, S. CA CDF Collaboration TI Search for a low-mass neutral Higgs boson with suppressed couplings to fermions using events with multiphoton final states SO PHYSICAL REVIEW D LA English DT Article ID FERMIOPHOBIC HIGGS; ATLAS DETECTOR; COLLISIONS; SIGNATURES; LHC; TEV AB A search for a Higgs boson with suppressed couplings to fermions, h(f), assumed to be the neutral, lower-mass partner of the Higgs boson discovered at the Large Hadron Collider, is reported. Such a Higgs boson could exist in extensions of the standard model with two Higgs doublets, and could be produced via p (p) over bar -> H(+/-)h(f) -> W*h(f)h(f) -> 4 gamma + X where H (+/-) is a charged Higgs boson. This analysis uses all events withat least three photons in the final state from proton-antiproton collisions at a center-of-mass energy of 1.96 TeV collected by the Collider Detector at Fermilab, corresponding to an integrated luminosity of 9.2 fb(-1). No evidence of a signal is observed in the data. 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[Dorigo, M.] Univ Trieste, I-34127 Trieste, Italy. [Hara, K.; Kim, S. H.; Kurata, M.; Miyake, H.; Nagai, Y.; Sato, K.; Shimojima, M.; Sudo, Y.; Takemasa, K.; Takeuchi, Y.; Tomura, T.; Ukegawa, F.] Univ Tsukuba, Tsukuba, Ibaraki 305, Japan. [Hare, M.; Napier, A.; Rolli, S.; Sliwa, K.] Tufts Univ, Medford, MA 02155 USA. [Arisawa, T.; Ebina, K.; Funakoshi, Y.; Kimura, N.; Kondo, K.; Naganoma, J.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo 169, Japan. [Clarke, C.; Harr, R. F.; Karchin, P. E.; Mattson, M. E.] Wayne State Univ, Detroit, MI 48201 USA. [Bellinger, J.; Carlsmith, D.; Herndon, M.; Parker, W.; Pondrom, L.] Univ Wisconsin, Madison, WI 53706 USA. [Husemann, U.; Lockwitz, S.; Loginov, A.] Yale Univ, New Haven, CT 06520 USA. RP Aaltonen, T (reprint author), Univ Helsinki, Dept Phys, Div High Energy Phys, FIN-00014 Helsinki, Finland. RI Prokoshin, Fedor/E-2795-2012; Canelli, Florencia/O-9693-2016; Ruiz, Alberto/E-4473-2011; Paulini, Manfred/N-7794-2014; OI Prokoshin, Fedor/0000-0001-6389-5399; Canelli, Florencia/0000-0001-6361-2117; Ruiz, Alberto/0000-0002-3639-0368; Paulini, Manfred/0000-0002-6714-5787; Farrington, Sinead/0000-0001-5350-9271; Robson, Aidan/0000-0002-1659-8284; Dorigo, Mirco/0000-0002-0681-6946; Brucken, Jens Erik/0000-0001-6066-8756; Torre, Stefano/0000-0002-7565-0118 FU U.S. Department of Energy; National Science Foundation; Italian Istituto Nazionale di Fisica Nucleare; Ministry of Education, Culture, Sports, Science and Technology of Japan; Natural Sciences and Engineering Research Council of Canada; National Science Council of the Republic of China; Swiss National Science Foundation; A. P. Sloan Foundation; Bundesministerium fur Bildung und Forschung, Germany; Korean World Class University Program; National Research Foundation of Korea; Science and Technology Facilities Council, United Kingdom; Royal Society, United Kingdom; Russian Foundation for Basic Research; Ministerio de Ciencia e Innovacion, and Programa Consolider-Ingenio, Spain; Slovak RD Agency; Academy of Finland; Australian Research Council (ARC); EU community Marie Curie Fellowship [302103] FX We thank the Fermilab staff and the technical staffs of the participating institutions for their vital contributions. This work was supported by the U.S. Department of Energy and National Science Foundation; the Italian Istituto Nazionale di Fisica Nucleare; the Ministry of Education, Culture, Sports, Science and Technology of Japan; the Natural Sciences and Engineering Research Council of Canada; the National Science Council of the Republic of China; the Swiss National Science Foundation; the A. P. Sloan Foundation; the Bundesministerium fur Bildung und Forschung, Germany; the Korean World Class University Program, the National Research Foundation of Korea; the Science and Technology Facilities Council and the Royal Society, United Kingdom; the Russian Foundation for Basic Research; the Ministerio de Ciencia e Innovacion, and Programa Consolider-Ingenio 2010, Spain; the Slovak R&D Agency; the Academy of Finland; the Australian Research Council (ARC); and the EU community Marie Curie Fellowship Contract No. 302103. NR 38 TC 0 Z9 0 U1 7 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JUN 20 PY 2016 VL 93 IS 11 AR 112010 DI 10.1103/PhysRevD.93.112010 PG 8 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DP0TY UT WOS:000378203800002 ER PT J AU Accardi, A Brady, LT Melnitchouk, W Owens, JF Sato, N AF Accardi, A. Brady, L. T. Melnitchouk, W. Owens, J. F. Sato, N. TI Constraints on large-x parton distributions from new weak boson production and deep-inelastic scattering data SO PHYSICAL REVIEW D LA English DT Article ID DEUTERON STRUCTURE FUNCTIONS; NUCLEAR-STRUCTURE FUNCTIONS; NEUTRON STRUCTURE; CROSS-SECTIONS; HEAVY QUARKS; QCD ANALYSIS; PROTON; EMC; MODEL; PDFS AB We present a new set of leading-twist parton distribution functions, referred to as "CJ15," which take advantage of developments in the theoretical treatment of nuclear corrections as well as new data. The analysis includes, for the first time, data on the free neutron structure function from Jefferson Lab and new high-precision charged lepton and W-boson asymmetry data from Fermilab. These significantly reduce the uncertainty on the d/u ratio at large values of x and provide new insights into the partonic structure of bound nucleons. C1 [Accardi, A.] Hampton Univ, Hampton, VA 23668 USA. [Accardi, A.; Brady, L. T.; Melnitchouk, W.; Sato, N.] Jefferson Lab, Newport News, VA 23606 USA. [Brady, L. T.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Owens, J. F.] Florida State Univ, Tallahassee, FL 32306 USA. RP Accardi, A (reprint author), Hampton Univ, Hampton, VA 23668 USA. FU DOE [DE-AC05-06OR23177, DE-FG02-97ER41922, DE-SC0008791] FX We thank E. Christy, C. Keppel, P. Monaghan and S. Malace for their collaboration and assistance with the experimental data sets and S. Kulagin and R. Petti for helpful discussions. This work was supported by the DOE Contract No. DE-AC05-06OR23177, under which Jefferson Science Associates, LLC operates Jefferson Lab. The work of J.F.O. and A. A. was supported in part by DOE Contracts No. DE-FG02-97ER41922 and No. DE-SC0008791, respectively. NR 110 TC 10 Z9 10 U1 4 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JUN 20 PY 2016 VL 93 IS 11 AR 114017 DI 10.1103/PhysRevD.93.114017 PG 21 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DP0TY UT WOS:000378203800004 ER PT J AU King, Z Pal, B Schwartz, AJ Adachi, I Aihara, H Al Said, S Asner, DM Atmacan, H Aushev, T Ayad, R Bakich, AM Behera, P Bhardwaj, V Bhuyan, B Biswal, J Bobrov, A Bozek, A Browder, TE Cervenkov, D Chekelian, V Cheon, BG Chilikin, K Chistov, R Cho, K Chobanova, V Choi, Y Cinabro, D Dalseno, J Dash, N Dolezal, Z Dutta, D Eidelman, S Farhat, H Ferber, T Fulsom, BG Gaur, V Gabyshev, N Garmash, A Gillard, R Glattauer, R Goh, YM Goldenzweig, P Golob, B Haba, J Hara, T Hayasaka, K Hayashii, H Horiguchi, T Hou, WS Hsu, CL Iijima, T Inami, K Inguglia, G Ishikawa, A Itoh, R Iwasaki, Y Jacobs, WW Jeon, HB Joo, KK Julius, T Kang, KH Kato, E Kawasaki, T Kiesling, C Kim, DY Kim, HJ Kim, JB Kim, KT Kim, SH Kim, YJ Kinoshita, K Kodys, P Korpar, S Kotchetkov, D Krizan, P Krokovny, P Kuhr, T Kumita, T Lee, IS Li, CH Li, H Li, L Li, Y Gioi, LL Libby, J Luo, T Masuda, M Matsuda, T Matvienko, D Miyabayashi, K Miyata, H Mizuk, R Mohanty, GB Moll, A Nakao, M Nakazawa, H Nanut, T Nath, KJ Negishi, K Nishida, S Ogawa, S Okuno, S Ostrowicz, W Park, CW Paul, S Pedlar, TK Pesantez, L Pestotnik, R Petric, M Piilonen, LE Pulvermacher, C Rauch, J Ritter, M Rostomyan, A Ryu, S Sahoo, H Sakai, Y Sandilya, S Santelj, L Sanuki, T Sato, Y Savinov, V Schluter, T Schneider, O Schnell, G Schwanda, C Seino, Y Senyo, K Sevior, ME Shebalin, V Shen, CP Shibata, TA Shiu, JG Shwartz, B Simon, F Solovieva, E Stanic, S Staric, M Strube, JF Stypula, J Sumihama, M Takizawa, M Taniguchi, N Teramoto, Y Trabelsi, K Uchida, M Uglov, T Unno, Y Uno, S Urquijo, P Usov, Y Vanhoefer, P Varner, G Varvell, KE Vorobyev, V Wang, CH Wang, MZ Wang, P Watanabe, M Watanabe, Y Wehle, S Williams, KM Won, E Yamaoka, J Yashchenko, S Yook, Y Yuan, CZ Zhang, ZP Zhilich, V Zupanc, A AF King, Z. Pal, B. Schwartz, A. J. Adachi, I. Aihara, H. Al Said, S. Asner, D. M. Atmacan, H. Aushev, T. Ayad, R. Bakich, A. M. Behera, P. Bhardwaj, V. Bhuyan, B. Biswal, J. Bobrov, A. Bozek, A. Browder, T. E. Cervenkov, D. Chekelian, V. Cheon, B. G. Chilikin, K. Chistov, R. Cho, K. Chobanova, V. Choi, Y. Cinabro, D. Dalseno, J. Dash, N. Dolezal, Z. Dutta, D. Eidelman, S. Farhat, H. Ferber, T. Fulsom, B. G. Gaur, V. Gabyshev, N. Garmash, A. Gillard, R. Glattauer, R. Goh, Y. M. Goldenzweig, P. Golob, B. Haba, J. Hara, T. Hayasaka, K. Hayashii, H. Horiguchi, T. Hou, W. -S. Hsu, C. -L. Iijima, T. Inami, K. Inguglia, G. Ishikawa, A. Itoh, R. Iwasaki, Y. Jacobs, W. W. Jeon, H. B. Joo, K. K. Julius, T. Kang, K. H. Kato, E. Kawasaki, T. Kiesling, C. Kim, D. Y. Kim, H. J. Kim, J. B. Kim, K. T. Kim, S. H. Kim, Y. J. Kinoshita, K. Kodys, P. Korpar, S. Kotchetkov, D. Krizan, P. Krokovny, P. Kuhr, T. Kumita, T. Lee, I. S. Li, C. H. Li, H. Li, L. Li, Y. Gioi, L. Li Libby, J. Luo, T. Masuda, M. Matsuda, T. Matvienko, D. Miyabayashi, K. Miyata, H. Mizuk, R. Mohanty, G. B. Moll, A. Nakao, M. Nakazawa, H. Nanut, T. Nath, K. J. Negishi, K. Nishida, S. Ogawa, S. Okuno, S. Ostrowicz, W. Park, C. W. Paul, S. Pedlar, T. K. Pesantez, L. Pestotnik, R. Petric, M. Piilonen, L. E. Pulvermacher, C. Rauch, J. Ritter, M. Rostomyan, A. Ryu, S. Sahoo, H. Sakai, Y. Sandilya, S. Santelj, L. Sanuki, T. Sato, Y. Savinov, V. Schlueter, T. Schneider, O. Schnell, G. Schwanda, C. Seino, Y. Senyo, K. Sevior, M. E. Shebalin, V. Shen, C. P. Shibata, T. -A. Shiu, J. -G. Shwartz, B. Simon, F. Solovieva, E. Stanic, S. Staric, M. Strube, J. F. Stypula, J. Sumihama, M. Takizawa, M. Taniguchi, N. Teramoto, Y. Trabelsi, K. Uchida, M. Uglov, T. Unno, Y. Uno, S. Urquijo, P. Usov, Y. Vanhoefer, P. Varner, G. Varvell, K. E. Vorobyev, V. Wang, C. H. Wang, M. -Z. Wang, P. Watanabe, M. Watanabe, Y. Wehle, S. Williams, K. M. Won, E. Yamaoka, J. Yashchenko, S. Yook, Y. Yuan, C. Z. Zhang, Z. P. Zhilich, V. Zupanc, A. CA Belle Collaboration TI Search for the decay B-0 -> phi gamma SO PHYSICAL REVIEW D LA English DT Article ID CP-VIOLATION; BELLE; DETECTOR; PACKAGE AB We have searched for the decay B-0 -> phi gamma sing the full Belle data set of 772 x 10(6) B (B) over bar pairs collected at the gamma(4S) resonance with the Belle detector at the KEKB e(+)e(-) collider. No signal is observed, and we set an upper limit on the branching fraction of B(B-0 -> phi gamma) < 1.0 x 10(-7) at the 90% confidence level. This is the most stringent limit on this decay mode to date. C1 [Schnell, G.] Univ Basque Country UPV EHU, Bilbao 48080, Spain. [Shen, C. P.] Beihang Univ, Beijing 100191, Peoples R China. [Pesantez, L.] Univ Bonn, D-53115 Bonn, Germany. [Bobrov, A.; Eidelman, S.; Gabyshev, N.; Garmash, A.; Krokovny, P.; Matvienko, D.; Shebalin, V.; Shwartz, B.; Usov, Y.; Vorobyev, V.; Zhilich, V.] RAS, Budker Inst Nucl Phys, SB, Novosibirsk 630090, Russia. [Cervenkov, D.; Dolezal, Z.; Kodys, P.] Charles Univ Prague, Fac Math & Phys, CR-12116 Prague, Czech Republic. [Joo, K. K.] Chonnam Natl Univ, Kwangju 660701, South Korea. [King, Z.; Pal, B.; Schwartz, A. J.; Kinoshita, K.] Univ Cincinnati, Cincinnati, OH 45221 USA. [Ferber, T.; Inguglia, G.; Rostomyan, A.; Wehle, S.; Yashchenko, S.] DESY, D-22607 Hamburg, Germany. [Sumihama, M.] Gifu Univ, Gifu 5011193, Japan. [Adachi, I.; Haba, J.; Hara, T.; Itoh, R.; Nakao, M.; Nishida, S.; Sakai, Y.; Trabelsi, K.; Uno, S.] SOKENDAI Grad Univ Adv Studies, Hayama 2400193, Japan. [Cheon, B. G.; Goh, Y. M.; Kim, S. H.; Lee, I. S.; Unno, Y.] Hanyang Univ, Seoul 133791, South Korea. [Browder, T. E.; Kotchetkov, D.; Sahoo, H.; Varner, G.] Univ Hawaii, Honolulu, HI 96822 USA. [Adachi, I.; Haba, J.; Hara, T.; Itoh, R.; Iwasaki, Y.; Nakao, M.; Nishida, S.; Sakai, Y.; Santelj, L.; Taniguchi, N.; Trabelsi, K.; Uno, S.] KEK, High Energy Accelerator Res Org, Tsukuba, Ibaraki 3050801, Japan. [Schnell, G.] Ikerbasque, Basque Fdn Sci, Bilbao 48013, Spain. [Dash, N.] Indian Inst Technol, Bhubaneswar 751007, Orissa, India. [Bhuyan, B.; Nath, K. J.] Indian Inst Technol Guwahati, Gauhati 781039, Assam, India. [Behera, P.; Libby, J.] Indian Inst Technol, Chennai 600036, Tamil Nadu, India. [Jacobs, W. W.; Li, H.] Indiana Univ, Bloomington, IN 47408 USA. [Wang, P.; Yuan, C. Z.] Chinese Acad Sci, Inst High Energy Phys, Beijing 100049, Peoples R China. [Glattauer, R.; Schwanda, C.] Inst High Energy Phys, A-1050 Vienna, Austria. [Biswal, J.; Golob, B.; Korpar, S.; Krizan, P.; Nanut, T.; Pestotnik, R.; Petric, M.; Staric, M.; Zupanc, A.] J Stefan Inst, Ljubljana 1000, Slovenia. [Okuno, S.; Watanabe, Y.] Kanagawa Univ, Yokohama, Kanagawa 2218686, Japan. [Goldenzweig, P.; Pulvermacher, C.] Karlsruhe Inst Technol, Inst Expt Kernphys, D-76131 Karlsruhe, Germany. [Al Said, S.] King Abdulaziz Univ, Fac Sci, Dept Phys, Jeddah 21589, Saudi Arabia. [Cho, K.; Kim, Y. J.] Korea Inst Sci & Technol Informat, Daejeon 305806, South Korea. [Kim, J. B.; Kim, K. T.; Won, E.] Korea Univ, Seoul 136713, South Korea. [Jeon, H. B.; Kang, K. H.; Kim, H. J.] Kyungpook Natl Univ, Taegu 702701, South Korea. [Schneider, O.] Ecole Polytech Fed Lausanne, CH-1015 Lausanne, Switzerland. [Chilikin, K.; Chistov, R.; Mizuk, R.; Solovieva, E.; Uglov, T.] Russian Acad Sci, PN Lebedev Phys Inst, Moscow 119991, Russia. [Golob, B.; Krizan, P.; Zupanc, A.] Univ Ljubljana, Fac Math & Phys, Ljubljana 1000, Slovenia. [Kuhr, T.; Ritter, M.; Schlueter, T.] Univ Munich, Marchioninistr 15, D-80539 Munich, Germany. [Korpar, S.] Univ Maribor, SLO-2000 Maribor, Slovenia. [Chekelian, V.; Chobanova, V.; Dalseno, J.; Kiesling, C.; Gioi, L. Li; Moll, A.; Simon, F.; Vanhoefer, P.] Max Planck Inst Phys & Astrophys, D-80805 Munich, Germany. [Hsu, C. -L.; Julius, T.; Li, C. H.; Sevior, M. E.; Urquijo, P.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Atmacan, H.] Middle E Tech Univ, TR-06531 Ankara, Turkey. [Chilikin, K.; Chistov, R.; Mizuk, R.] Moscow Phys Engn Inst, Moscow 115409, Russia. [Aushev, T.; Mizuk, R.; Solovieva, E.; Uglov, T.] Moscow Inst Phys & Technol, Dolgoprudnyi 141700, Moscow Region, Russia. [Iijima, T.; Inami, K.; Sato, Y.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648602, Japan. [Hayasaka, K.; Iijima, T.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648602, Japan. [Hayashii, H.; Miyabayashi, K.] Nara Womens Univ, Nara 6308506, Japan. [Wang, C. H.] Natl United Univ, Miaoli 36003, Taiwan. [Hou, W. -S.; Shiu, J. -G.; Wang, M. -Z.] Natl Taiwan Univ, Dept Phys, Taipei 10617, Taiwan. [Bozek, A.; Ostrowicz, W.; Stypula, J.] H Niewodniczanski Inst Nucl Phys, PL-31342 Krakow, Poland. [Kawasaki, T.; Miyata, H.; Seino, Y.; Watanabe, M.] Niigata Univ, Niigata 9502181, Japan. [Stanic, S.] Univ Nova Gor, Nova Gorica 5000, Slovenia. [Bobrov, A.; Eidelman, S.; Gabyshev, N.; Garmash, A.; Krokovny, P.; Matvienko, D.; Shebalin, V.; Shwartz, B.; Usov, Y.; Vorobyev, V.; Zhilich, V.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Teramoto, Y.] Osaka City Univ, Osaka 5588585, Japan. [Asner, D. M.; Fulsom, B. G.; Strube, J. F.; Yamaoka, J.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Luo, T.; Savinov, V.] Univ Pittsburgh, Pittsburgh, PA 15260 USA. [Li, L.; Zhang, Z. P.] Univ Sci & Technol China, Hefei 230026, Peoples R China. [Ryu, S.] Seoul Natl Univ, Seoul 151742, South Korea. [Takizawa, M.] Showa Pharmaceut Univ, Tokyo 1948543, Japan. [Kim, D. Y.] Soongsil Univ, Seoul 156743, South Korea. [Bhardwaj, V.] Univ S Carolina, Columbia, SC 29208 USA. [Choi, Y.; Park, C. W.] Sungkyunkwan Univ, Suwon 440746, South Korea. [Bakich, A. M.; Varvell, K. E.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Al Said, S.; Ayad, R.] Univ Tabuk, Fac Sci, Dept Phys, Tabuk 71451, Saudi Arabia. [Dutta, D.; Gaur, V.; Mohanty, G. B.; Sandilya, S.] Tata Inst Fundamental Res, Homi Bhabha Rd, Mumbai 400005, Maharashtra, India. [Dalseno, J.; Moll, A.; Simon, F.] Tech Univ Munich, Excellence Cluster Univ, D-85748 Garching, Germany. [Paul, S.; Rauch, J.] Tech Univ Munich, Dept Phys, D-85748 Garching, Germany. [Ogawa, S.] Toho Univ, Funabashi, Chiba 2748510, Japan. [Horiguchi, T.; Ishikawa, A.; Kato, E.; Negishi, K.; Sanuki, T.] Tohoku Univ, Dept Phys, Sendai, Miyagi 9808578, Japan. [Masuda, M.] Univ Tokyo, Earthquake Res Inst, Tokyo 1130032, Japan. [Aihara, H.] Univ Tokyo, Dept Phys, Tokyo 1130033, Japan. [Shibata, T. -A.; Uchida, M.] Tokyo Inst Technol, Tokyo 1528550, Japan. [Kumita, T.] Tokyo Metropolitan Univ, Tokyo 1920397, Japan. [Li, Y.; Piilonen, L. E.; Williams, K. M.] Virginia Polytech Inst & State Univ, CNP, Blacksburg, VA 24061 USA. [Cinabro, D.; Farhat, H.; Gillard, R.] Wayne State Univ, Detroit, MI 48202 USA. [Senyo, K.] Yamagata Univ, Yamagata 9908560, Japan. [Yook, Y.] Yonsei Univ, Seoul 120749, South Korea. [Matsuda, T.] Miyazaki Univ, Miyazaki 8892192, Japan. [Nakazawa, H.] Natl Cent Univ, Chungli 32054, Taiwan. [Pedlar, T. K.] Luther Coll, Decorah, IA 52101 USA. RP King, Z (reprint author), Univ Cincinnati, Cincinnati, OH 45221 USA. RI Paul, Stephan/K-9237-2016; Aihara, Hiroaki/F-3854-2010; Uglov, Timofey/B-2406-2014; Chilikin, Kirill/B-4402-2014; Chistov, Ruslan/B-4893-2014; Mizuk, Roman/B-3751-2014; Cervenkov, Daniel/D-2884-2017; Faculty of, Sciences, KAU/E-7305-2017; Solovieva, Elena/B-2449-2014; OI Paul, Stephan/0000-0002-8813-0437; Aihara, Hiroaki/0000-0002-1907-5964; Uglov, Timofey/0000-0002-4944-1830; Chilikin, Kirill/0000-0001-7620-2053; Chistov, Ruslan/0000-0003-1439-8390; Cervenkov, Daniel/0000-0002-1865-741X; Solovieva, Elena/0000-0002-5735-4059; Inguglia, Gianluca/0000-0003-0331-8279 FU Ministry of Education, Culture, Sports, Science, and Technology (MEXT) of Japan; Japan Society for the Promotion of Science (JSPS); Tau-Lepton Physics Research Center of Nagoya University; Australian Research Council; Austrian Science Fund [P 22742-N16, P 26794-N20]; National Natural Science Foundation of China [10575109, 10775142, 10875115, 11175187, 11475187, 11575017]; Chinese Academy of Science Center for Excellence in Particle Physics; Ministry of Education, Youth and Sports of the Czech Republic [LG14034]; Carl Zeiss Foundation; Deutsche Forschungsgemeinschaft; Excellence Cluster Universe; Volkswagen-Stiftung; Department of Science and Technology of India; Istituto Nazionale di Fisica Nucleare of Italy; WCU program of the Ministry of Education, National Research Foundation (NRF) of Korea [2011-0029457, 2012-0008143, 2012R1A1A2008330, 2013R1A1A3007772, 2014R1A2A2A01005286, 2014R1A2A2A01002734, 2015R1A2A2A01003280, 2015H1A2A1033649]; Basic Research Lab program under NRF Grant [KRF-2011-0020333]; Brain Korea 21-Plus program and Radiation Science Research Institute; Polish Ministry of Science and Higher Education; National Science Center; Ministry of Education and Science of the Russian Federation; Russian Foundation for Basic Research; Slovenian Research Agency; Ikerbasque, Basque Foundation for Science; Euskal Herriko Unibertsitatea (UPV/EHU) (Spain) [UFI 11/55]; Swiss National Science Foundation; Ministry of Education; Ministry of Science and Technology of Taiwan; U.S. Department of Energy; National Science Foundation; MEXT for Science Research in a Priority Area ("New Development of Flavor Physics"); JSPS for Creative Scientific Research ("Evolution of Tau-lepton Physics"); [NRF-2013K1A3A7A06056592] FX We thank the KEKB group for the excellent operation of the accelerator; the KEK cryogenics group for the efficient operation of the solenoid; and the KEK computer group, the National Institute of Informatics, and the PNNL/EMSL computing group for valuable computing and SINET4 network support. We acknowledge support from the Ministry of Education, Culture, Sports, Science, and Technology (MEXT) of Japan, the Japan Society for the Promotion of Science (JSPS), and the Tau-Lepton Physics Research Center of Nagoya University; the Australian Research Council; Austrian Science Fund under Grant No. P 22742-N16 and P 26794-N20; the National Natural Science Foundation of China under Contracts No. 10575109, No. 10775142, No. 10875115, No. 11175187, No. 11475187 and No. 11575017; the Chinese Academy of Science Center for Excellence in Particle Physics; the Ministry of Education, Youth and Sports of the Czech Republic under Contract No. LG14034; the Carl Zeiss Foundation, the Deutsche Forschungsgemeinschaft, the Excellence Cluster Universe, and the Volkswagen-Stiftung; the Department of Science and Technology of India; the Istituto Nazionale di Fisica Nucleare of Italy; the WCU program of the Ministry of Education, National Research Foundation (NRF) of Korea Grants No. 2011-0029457, No. 2012-0008143, No. 2012R1A1A2008330, No. 2013R1A1A3007772, No. 2014R1A2A2A01005286, No. 2014R1A2A2A01002734, No. 2015R1A2A2A01003280, No. 2015H1A2A1033649; the Basic Research Lab program under NRF Grant No. KRF-2011-0020333, Center for Korean J-PARC Users, No. NRF-2013K1A3A7A06056592; the Brain Korea 21-Plus program and Radiation Science Research Institute; the Polish Ministry of Science and Higher Education and the National Science Center; the Ministry of Education and Science of the Russian Federation and the Russian Foundation for Basic Research; the Slovenian Research Agency; Ikerbasque, Basque Foundation for Science and the Euskal Herriko Unibertsitatea (UPV/EHU) under program UFI 11/55 (Spain); the Swiss National Science Foundation; the Ministry of Education and the Ministry of Science and Technology of Taiwan; and the U.S. Department of Energy and the National Science Foundation. This work is supported by a Grant-in-Aid from MEXT for Science Research in a Priority Area ("New Development of Flavor Physics") and from JSPS for Creative Scientific Research ("Evolution of Tau-lepton Physics"). NR 24 TC 0 Z9 0 U1 4 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JUN 20 PY 2016 VL 93 IS 11 AR 111101 DI 10.1103/PhysRevD.93.111101 PG 6 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DP0TY UT WOS:000378203800001 ER PT J AU Sadofyev, AV Yin, Y AF Sadofyev, Andrey V. Yin, Yi TI Drag suppression in anomalous chiral media SO PHYSICAL REVIEW D LA English DT Article ID HEAVY-ION COLLISIONS; WEYL FERMIONS; SUPERFLUIDITY; VIOLATION; TRANSPORT AB We study a heavy impurity moving longitudinal with the direction of an external magnetic field in an anomalous chiral medium. Such system would carry a nondissipative current of chiral magnetic effect associated with the anomaly. We show, by generalizing Landau's criterion for superfluidity, that the "anomalous component" which gives rise to the anomalous transport will not contribute to the drag experienced by an impurity. We argue on a very general basis that those systems with a strong magnetic field would exhibit an interesting transport phenomenon-the motion of the heavy impurity is frictionless, in analogy to the case of a superfluid. We demonstrate and confirm our general results with two complementary examples: weakly coupled chiral fermion gases and strongly interacting chiral liquids. C1 [Sadofyev, Andrey V.] MIT, Ctr Theoret Phys, Cambridge, MA 02139 USA. [Sadofyev, Andrey V.] ITEP, B Cheremushkinskaya 25, Moscow 117218, Russia. [Yin, Yi] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. RP Sadofyev, AV (reprint author), MIT, Ctr Theoret Phys, Cambridge, MA 02139 USA.; Sadofyev, AV (reprint author), ITEP, B Cheremushkinskaya 25, Moscow 117218, Russia. EM sadofyev@mit.edu; yyin@bnl.gov FU DOE [DE-SC0012704, DE-SC0011090]; Russian Science Foundation [16-12-10059] FX The authors would like to thank K. Rajagopal, M. Stephanov, Naoki Yamamoto for very helpful comments on the draft and K. Fukushima, J. Goldstone, K. Hattori, R. Jackiw, D. Kharzeev, L. McLerran, F. Wilczek, Ho-Ung. Yee, V. I. Zakharov for useful conversations. We also thank the referees for providing constructive comments and help in improving the presentations of this paper. The work of Y. Y. was supported by DOE Contract No. DE-SC0012704. The part of the work of A. S. (Secs. III and IV) was supported by Russian Science Foundation Grant No 16-12-10059, the remaining part of the work of A. S. was supported by DOE Contract No. DE-SC0011090. NR 40 TC 3 Z9 3 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JUN 20 PY 2016 VL 93 IS 12 AR 125026 DI 10.1103/PhysRevD.93.125026 PG 6 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DP0UF UT WOS:000378204700011 ER PT J AU Deng, XY Haule, K Kotliar, G AF Deng, Xiaoyu Haule, Kristjan Kotliar, Gabriel TI Transport Properties of Metallic Ruthenates: A DFT plus DMFT Investigation SO PHYSICAL REVIEW LETTERS LA English DT Article ID HIGH-TEMPERATURE RESISTIVITY; FERMI-LIQUID BEHAVIOR; IOFFE-REGEL LIMIT; MEAN-FIELD THEORY; THERMODYNAMIC PROPERTIES; SUPERCONDUCTOR SR2RUO4; ELECTRONIC-STRUCTURE; SINGLE-CRYSTALS; STATE; CONDUCTIVITY AB We present a systematical theoretical study on the transport properties of an archetypal family of Hund's metals, Sr2RuO4, Sr3Ru2O7, SrRuO3, and CaRuO3, within the combination of first principles density functional theory and dynamical mean field theory. The agreement between theory and experiments for optical conductivity and resistivity is good, which indicates that electron-electron scattering dominates the transport of ruthenates. We demonstrate that in the single-site dynamical mean field approach the transport properties of Hund's metals fall into the scenario of "resilient quasiparticles." We explain why the single layered compound Sr2RuO4 has a relative weak correlation with respect to its siblings, which corroborates its good metallicity. C1 [Deng, Xiaoyu; Haule, Kristjan; Kotliar, Gabriel] Rutgers State Univ, Dept Phys & Astron, POB 849, Piscataway, NJ 08854 USA. [Kotliar, Gabriel] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RP Deng, XY (reprint author), Rutgers State Univ, Dept Phys & Astron, POB 849, Piscataway, NJ 08854 USA. RI Deng, Xiaoyu/F-2322-2015 OI Deng, Xiaoyu/0000-0001-7802-0966 FU NSF [DMR-1308141, DMR 1405303] FX We thank A. Georges and J. Mravlje for very useful discussions. We acknowledge support by NSF Grant No. DMR-1308141 (X. D. and G. K.) and NSF Grant No. DMR 1405303 (K. H.). NR 54 TC 2 Z9 2 U1 15 U2 28 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUN 20 PY 2016 VL 116 IS 25 AR 256401 DI 10.1103/PhysRevLett.116.256401 PG 6 WC Physics, Multidisciplinary SC Physics GA DP0VP UT WOS:000378208800004 PM 27391734 ER PT J AU Hawreliak, JA Lind, J Maddox, B Barham, M Messner, M Barton, N Jensen, BJ Kumar, M AF Hawreliak, J. A. Lind, J. Maddox, B. Barham, M. Messner, M. Barton, N. Jensen, B. J. Kumar, M. TI Dynamic Behavior of Engineered Lattice Materials SO SCIENTIFIC REPORTS LA English DT Article ID FOAMS AB Additive manufacturing (AM) is enabling the fabrication of materials with engineered lattice structures at the micron scale. These mesoscopic structures fall between the length scale associated with the organization of atoms and the scale at which macroscopic structures are constructed. Dynamic compression experiments were performed to study the emergence of behavior owing to the lattice periodicity in AM materials on length scales that approach a single unit cell. For the lattice structures, both bend and stretch dominated, elastic deflection of the structure was observed ahead of the compaction of the lattice, while no elastic deformation was observed to precede the compaction in a stochastic, random structure. The material showed lattice characteristics in the elastic response of the material, while the compaction was consistent with a model for compression of porous media. The experimental observations made on arrays of 4 x 4 x 6 lattice unit cells show excellent agreement with elastic wave velocity calculations for an infinite periodic lattice, as determined by Bloch wave analysis, and finite element simulations. C1 [Hawreliak, J. A.; Lind, J.; Maddox, B.; Barham, M.; Messner, M.; Barton, N.; Kumar, M.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Hawreliak, J. A.] Washington State Univ, Inst Shock Phys, Pullman, WA 99164 USA. [Jensen, B. J.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. RP Hawreliak, JA (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA.; Hawreliak, JA (reprint author), Washington State Univ, Inst Shock Phys, Pullman, WA 99164 USA. EM James.Hawreliak@wsu.edu FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Los Alamos National Laboratory (LANL) [DE-AC52-06NA25396]; Department of Energy, National Nuclear Security Administration [DE-NA0002442]; DOE Office of Science by Argonne National Laboratory [DE-AC02-06CH11357] FX Julie Jackson and Christopher Spadaccini (of LLNL) are gratefully acknowledged for supplying us with the samples tested in this study. C.T. Owens (LANL) is gratefully acknowledged for technical assistance with gun setup and shot execution. A.J. Iverson, C.A. Carlson, and M. Teel from National Security Technologies (NSTech) are thanked for their technical support in fielding of the X-ray PCI detector system. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344 and by Los Alamos National Laboratory (LANL) under contract DE-AC52-06NA25396. This publication is based in part upon work performed at the Dynamic Compression Sector at the Advanced Photon Source supported by the Department of Energy, National Nuclear Security Administration, under Award Number DE-NA0002442. This research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. NR 19 TC 1 Z9 1 U1 16 U2 35 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JUN 20 PY 2016 VL 6 AR 28094 DI 10.1038/srep28094 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DP1CJ UT WOS:000378227700001 PM 27321697 ER PT J AU Chen, CF Barai, P Smith, K Mukherjee, PP AF Chen, Chien-Fan Barai, Pallab Smith, Kandler Mukherjee, Partha P. TI Scaling Relations for Intercalation Induced Damage in Electrodes SO ELECTROCHIMICA ACTA LA English DT Article DE Lithium-ion battery electrode; mechanical degradation; scaling relation ID LITHIUM-ION BATTERIES; DIFFUSION-INDUCED STRESSES; REDUCED-ORDER MODEL; LI-ION; MECHANICAL DEGRADATION; CRYSTALLINE SOLIDS; IMPEDANCE RESPONSE; PARTICLES; FRACTURE; FRAGMENTATION AB Mechanical degradation, owing to intercalation induced stress and microcrack formation, is a key contributor to the electrode performance decay in lithium-ion batteries (LIBs). The stress generation and formation of microcracks are caused by the solid state diffusion of lithium in the active particles. In this work, scaling relations are constructed for diffusion induced damage in intercalation electrodes based on an extensive set of numerical experiments with a particle -level description of microcrack formation under disparate operating and cycling conditions, such as temperature, particle size, C-rate, and drive cycle. The microcrack formation and evolution in active particles is simulated based on a stochastic methodology. A reduced order scaling law is constructed based on an extensive set of data from the numerical experiments. The scaling relations include combinatorial constructs of concentration gradient, cumulative strain energy, and microcrack formation. The reduced order relations are further employed to study the influence of mechanical degradation on cell performance and validated against the high order model for the case of damage evolution during variable current vehicle drive cycle profiles. 2016 Elsevier Ltd. All rights reserved. C1 [Chen, Chien-Fan; Barai, Pallab; Mukherjee, Partha P.] Texas A&M Univ, Dept Mech Engn, College Stn, TX 77843 USA. [Smith, Kandler] Natl Renewable Energy Lab, Golden, CO USA. RP Mukherjee, PP (reprint author), Texas A&M Univ, Dept Mech Engn, College Stn, TX 77843 USA. EM pmukherjee@tamu.edu FU National Renewable Energy Laboratory (NREL); U.S. Department of Energy, Vehicles Technologies Office, Energy Storage Program FX Financial support from National Renewable Energy Laboratory (NREL) as a research contract to Texas A&M University is gratefully acknowledged. KS acknowledges funding provided by the U.S. Department of Energy, Vehicles Technologies Office, Energy Storage Program (program manager, Brian Cunningham). Assistance from Eric Wood at NREL for providing vehicle drive cycle profiles and from Bhaskar Vajipeyajula at Texas A&M University at the initial stage of this work are also gratefully acknowledged. NR 56 TC 3 Z9 3 U1 5 U2 18 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0013-4686 EI 1873-3859 J9 ELECTROCHIM ACTA JI Electrochim. Acta PD JUN 20 PY 2016 VL 204 BP 31 EP 49 DI 10.1016/j.electacta.2016.03.106 PG 19 WC Electrochemistry SC Electrochemistry GA DM1WD UT WOS:000376136700004 ER PT J AU Kim, Y Joachimiak, G Bigelow, L Babnigg, G Joachimiak, A AF Kim, Youngchang Joachimiak, Grazyna Bigelow, Lance Babnigg, Gyorgy Joachimiak, Andrzej TI How Aromatic Compounds Block DNA Binding of HcaR Catabolite Regulator SO JOURNAL OF BIOLOGICAL CHEMISTRY LA English DT Article ID 3-HYDROXYBENZOATE HYDROXYLASE GENE; COMAMONAS-TESTOSTERONI KH122-3S; CRYSTAL-STRUCTURE REVEALS; MARR FAMILY PROTEINS; SP STRAIN ADP1; TRANSCRIPTIONAL REGULATOR; ESCHERICHIA-COLI; HIGH-THROUGHPUT; DEINOCOCCUS-RADIODURANS; SULFOLOBUS-SOLFATARICUS AB Bacterial catabolism of aromatic compounds from various sources including phenylpropanoids and flavonoids that are abundant in soil plays an important role in the recycling of carbon in the ecosystem. We have determined the crystal structures of apo-HcaR from Acinetobacter sp. ADP1, a MarR/SlyA transcription factor, in complexes with hydroxycinnamates and a specific DNA operator. The protein regulates the expression of the hca catabolic operon in Acinetobacter and related bacterial strains, allowing utilization of hydroxycinnamates as sole sources of carbon. HcaR binds multiple ligands, and as a result the transcription of genes encoding several catabolic enzymes is increased. The 1.9-2.4 angstrom resolution structures presented here explain how HcaR recognizes four ligands (ferulate, 3,4-dihydroxybenzoate, p-coumarate, and vanillin) using the same binding site. The ligand promiscuity appears to be an adaptation to match a broad specificity of hydroxycinnamate catabolic enzymes while responding to toxic thioester intermediates. Structures of apo-HcaR and in complex with a specific DNA hca operator when combined with binding studies of hydroxycinnamates show how aromatic ligands render HcaR unproductive in recognizing a specific DNA target. The current study contributes to a better understanding of the hca catabolic operon regulation mechanism by the transcription factor HcaR. C1 [Kim, Youngchang; Joachimiak, Grazyna; Bigelow, Lance; Babnigg, Gyorgy; Joachimiak, Andrzej] Argonne Natl Lab, Midwest Ctr Struct Genom, 9700 S Cass Ave, Argonne, IL 60439 USA. [Kim, Youngchang; Babnigg, Gyorgy; Joachimiak, Andrzej] Argonne Natl Lab, Struct Biol Ctr, Biosci, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Joachimiak, A (reprint author), Argonne Natl Lab, Struct Biol Ctr, Biosci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM andrzejj@anl.gov FU National Institute of Health [GM115586, GM094585]; United States Department of Energy, Office of Biological and Environmental Research [DE-AC02-06CH11357] FX This work was supported by National Institute of Health Grants GM115586 and GM094585 and by United States Department of Energy, Office of Biological and Environmental Research, Contract DE-AC02-06CH11357. The authors declare that they have no conflicts of interest with the contents of this article. The content is solely the responsibility of the authors and does not necessarily represent the official views of the National Institutes of Health. NR 57 TC 0 Z9 0 U1 6 U2 6 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 0021-9258 EI 1083-351X J9 J BIOL CHEM JI J. Biol. Chem. PD JUN 17 PY 2016 VL 291 IS 25 BP 13243 EP 13256 DI 10.1074/jbc.M115.712067 PG 14 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA DR2YT UT WOS:000379770500029 PM 27129205 ER PT J AU Liu, JL Kim, JI Cusumano, JC Chapple, C Venugopalan, N Fischetti, RF Makowski, L AF Liu, Jiliang Kim, Jeong Im Cusumano, Joanne C. Chapple, Clint Venugopalan, Nagarajan Fischetti, Robert F. Makowski, Lee TI The impact of alterations in lignin deposition on cellulose organization of the plant cell wall SO BIOTECHNOLOGY FOR BIOFUELS LA English DT Article DE Lignin biosynthetic mutants; Cellulose fibril; X-ray microdiffraction ID ARABIDOPSIS-THALIANA; PHENYLPROPANOID PATHWAY; MONOMER COMPOSITION; MUTANTS DEFICIENT; BIOSYNTHESIS; FERULATE-5-HYDROXYLASE; MICRODIFFRACTION; MICROFIBRILS; ARCHITECTURE; COLLENCHYMA AB Background: Coordination of synthesis and assembly of the polymeric components of cell walls is essential for plant growth and development. Given the degree of co-mingling and cross-linking among cell wall components, cellulose organization must be dependent on the organization of other polymers such as lignin. Here we seek to identify aspects of that codependency by studying the structural organization of cellulose fibrils in stems from Arabidopsis plants harboring mutations in genes encoding enzymes involved in lignin biosynthesis. Plants containing high levels of G-lignin, S-lignin, H-lignin, aldehyde-rich lignin, and ferulic acid-containing lignin, along with plants with very low lignin content were grown and harvested and longitudinal sections of stem were prepared and dried. Scanning X-ray microdiffraction was carried out using a 5-micron beam that moved across the sections in 5-micron steps and complete diffraction patterns were collected at each raster point. Approximately, 16,000 diffraction patterns were analyzed to determine cellulose fibril orientation and order within the tissues making up the stems. Results: Several mutations-most notably those exhibiting (1) down-regulation of cinnamoyl CoA reductase which leads to cell walls deficient in lignin and (2) defect of cinnamic acid 4-hydroxylase which greatly reduces lignin content-exhibited significant decrease in the proportion of oriented cellulose fibrils in the cell wall. Distinctions between tissues were maintained in all variants and even in plants exhibiting dramatic changes in cellulosic order the trends between tissues (where apparent) were generally maintained. The resilience of cellulose to degradative processes was investigated by carrying out the same analysis on samples stored in water for 30 days prior to data collection. This treatment led to significant loss of cellulosic order in plants rich in aldehyde or H-lignin, less change in wild type, and essentially no change in samples with high levels of G-or S-lignin. Conclusions: These studies demonstrate that changes in lignin biosynthesis lead to significant disruption in the orientation and order of cellulose fibrils in all tissues of the stem. These dramatic phenotypic changes, in mutants with lignin rich in aldehyde or H-units, correlate with the impact the mutations have on the enzymatic degradation of the plant cell wall. C1 [Liu, Jiliang] Northeastern Univ, Dept Bioengn, 360 Huntington Ave, Boston, MA 02148 USA. [Kim, Jeong Im; Cusumano, Joanne C.; Chapple, Clint] Purdue Univ, Dept Biochem, 175 South Univ St, W Lafayette, IN 47907 USA. [Venugopalan, Nagarajan; Fischetti, Robert F.] Argonne Natl Lab, GM CA CAT, XSD, Adv Photon Source, 9700 Cass Ave, Lemont, IL 60439 USA. [Makowski, Lee] Northeastern Univ, Dept Chem & Chem Biol, 360 Huntington Ave, Boston, MA 02148 USA. RP Liu, JL (reprint author), Northeastern Univ, Dept Bioengn, 360 Huntington Ave, Boston, MA 02148 USA. EM liu.jil@husky.neu.edu FU Center for Direct Catalytic Conversion of Biomass to Biofuels (C3Bio), an Energy Frontier Research Center - U.S. department of Energy, Office of science, Basic Energy Science [DE-SC0000997]; U.S. DOE [DE-AC02-06CH11357]; National Institutes of Health, the National Cancer Institute [Y1-CO-1020]; National Institute of General Medical Science [Y1-GM-1104] FX This work was supported as part of the Center for Direct Catalytic Conversion of Biomass to Biofuels (C3Bio), an Energy Frontier Research Center funded by the U.S. department of Energy, Office of science, Basic Energy Science under Award #DE-SC0000997. Use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. DOE under Contract No. DE-AC02-06CH11357. Use of GM/CA at the APS was supported by the National Institutes of Health, the National Cancer Institute (Y1-CO-1020), and the National Institute of General Medical Science (Y1-GM-1104). NR 36 TC 1 Z9 1 U1 11 U2 17 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1754-6834 J9 BIOTECHNOL BIOFUELS JI Biotechnol. Biofuels PD JUN 17 PY 2016 VL 9 AR 126 DI 10.1186/s13068-016-0540-z PG 17 WC Biotechnology & Applied Microbiology; Energy & Fuels SC Biotechnology & Applied Microbiology; Energy & Fuels GA DQ0EF UT WOS:000378870500001 PM 27330560 ER PT J AU Aschenauer, EC D'Alesio, U Murgia, F AF Aschenauer, E. C. D'Alesio, U. Murgia, F. TI TMDs and SSAs in hadronic interactions SO EUROPEAN PHYSICAL JOURNAL A LA English DT Review ID SINGLE-SPIN ASYMMETRIES; TRANSVERSE-MOMENTUM DISTRIBUTION; DEEP-INELASTIC SCATTERING; DRELL-YAN PROCESSES; HARD-SCATTERING; PROCESS DEPENDENCE; STATE INTERACTIONS; PROTON COLLISIONS; PHOTON PRODUCTION; BOSON PRODUCTION AB We present an overview on the current experimental and phenomenological status of transverse single-spin asymmetries (tSSAs) in proton-proton collisions. In particular, we focus on large-pT inclusive pion, photon, jet, pion-jet production and Drell-Yan processes. For all of them theoretical estimates are given in terms of a generalised parton model (GPM) based on a transverse-momentum-dependent (TMD) factorisation scheme. Comparisons with the corresponding results in a collinear twist-3 formalism and in a modified GPM approach are also made. On the experimental side, a selection of the most interesting and recent results from RHIC is presented. C1 [Aschenauer, E. C.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [D'Alesio, U.] Univ Cagliari, Dipartimento Fis, I-09042 Monserrato, CA, Italy. [D'Alesio, U.; Murgia, F.] Ist Nazl Fis Nucl, Sez Cagliari, CP 170, I-09042 Monserrato, CA, Italy. RP D'Alesio, U (reprint author), Univ Cagliari, Dipartimento Fis, I-09042 Monserrato, CA, Italy.; D'Alesio, U (reprint author), Ist Nazl Fis Nucl, Sez Cagliari, CP 170, I-09042 Monserrato, CA, Italy. EM umberto.dalesio@ca.infn.it FU US Department of Energy [DE-SC0012704] FX ECA is grateful to her colleagues in the spin working groups of STAR and PHENIX. This work was supported by the US Department of Energy under Contract No. DE-SC0012704. UD and FM acknowledge the long and fruitful collaboration with M. Anselmino, M. Boglione, E. Leader, S. Melis, C. Pisano and A. Prokudin. NR 107 TC 3 Z9 3 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6001 EI 1434-601X J9 EUR PHYS J A JI Eur. Phys. J. A PD JUN 17 PY 2016 VL 52 IS 6 AR 156 DI 10.1140/epja/i2016-16156-4 PG 19 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA DP8NA UT WOS:000378753700004 ER PT J AU Rogers, TC AF Rogers, T. C. TI An overview of transverse-momentum-dependent factorization and evolution SO EUROPEAN PHYSICAL JOURNAL A LA English DT Review ID DEEP-INELASTIC SCATTERING; DRELL-YAN PROCESS; UNINTEGRATED PARTON DISTRIBUTIONS; PROTON-NUCLEUS COLLISIONS; INCLUSIVE PION-PRODUCTION; FINAL-STATE INTERACTIONS; SINGLE-SPIN ASYMMETRIES; VECTOR-BOSON PRODUCTION; ONE-LOOP CORRECTIONS; HADRON COLLIDERS AB I review TMD factorization and evolution theorems, with an emphasis on the treatment by Collins and originating in the Collins-Soper-Sterman (CSS) formalism. I summarize basic results while attempting to trace their development over that past several decades. C1 [Rogers, T. C.] Old Dominion Univ, Dept Phys, Norfolk, VA 23529 USA. [Rogers, T. C.] Jefferson Lab, Ctr Theory, 12000 Jefferson Ave, Newport News, VA 23606 USA. RP Rogers, TC (reprint author), Old Dominion Univ, Dept Phys, Norfolk, VA 23529 USA.; Rogers, TC (reprint author), Jefferson Lab, Ctr Theory, 12000 Jefferson Ave, Newport News, VA 23606 USA. EM trogers@jlab.org FU DOE [DE-AC05-06OR23177] FX I acknowledge many useful conversations with J. Collins who also provided suggestions on the text. I also thank C. Aidala, M. Diehl, and R. Fatemi for helpful comments on the text. This work was supported by the DOE contract No. DE-AC05-06OR23177, under which Jefferson Science Associates, LLC operates Jefferson Lab. NR 118 TC 7 Z9 7 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6001 EI 1434-601X J9 EUR PHYS J A JI Eur. Phys. J. A PD JUN 17 PY 2016 VL 52 IS 6 AR 153 DI 10.1140/epja/i2016-16153-7 PG 12 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA DP8NA UT WOS:000378753700001 ER PT J AU Yu, C Long, H Jin, YH Zhang, W AF Yu, Chao Long, Hai Jin, Yinghua Zhang, Wei TI Synthesis of Cyclic Porphyrin Trimers through Alkyne Metathesis Cyclooligomerization and Their Host-Guest Binding Study SO ORGANIC LETTERS LA English DT Article ID ARYLENE ETHYNYLENE MACROCYCLES; DYNAMIC COVALENT CHEMISTRY; LIGHT-HARVESTING COMPLEX; SUPRAMOLECULAR CHEMISTRY; CRYSTAL-STRUCTURE; ARYLENEETHYNYLENE CAGES; FULLERENES; CATALYSTS; ROUTES; DIMERS AB Cyclic porphyrin trimers were synthesized through one-step cyclooligomerization via alkyne metathesis from diyne monomers. These macrocydes show interesting host-guest binding interactions with fullerenes selectively binding C-70 (6 x 10(3) M-1) over C-60 and C-84 (no binding observed). The fullerene-encapsulated host-guest complex can undergo guest or host exchange in the presence of another guest (2,4,6-tri(4-pyridy1)-1,3,5-triazine) or host (cage COPS) molecule with higher binding affinity. C1 [Yu, Chao; Jin, Yinghua; Zhang, Wei] Univ Colorado, Dept Chem & Biochem, Campus Box 215, Boulder, CO 80309 USA. [Long, Hai] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Zhang, W (reprint author), Univ Colorado, Dept Chem & Biochem, Campus Box 215, Boulder, CO 80309 USA. EM wei.zhang@colorado.edu RI Long, Hai/C-5838-2015; Yu, Chao/H-4788-2015 OI Yu, Chao/0000-0001-8062-9498 FU National Science Foundation [DMR-1055705]; Office of Energy Efficiency and Renewable Energy of the U.S. Department of Energy [DE-AC36-08GO28308] FX We thank the National Science Foundation (DMR-1055705) for financial support and Dr. Richard K. Shoemaker (University of Colorado Boulder) for NMR assistance. This research used capabilities of the National Renewable Energy Laboratory Computational Sciences Center, which is supported by the Office of Energy Efficiency and Renewable Energy of the U.S. Department of Energy under Contract No. DE-AC36-08GO28308. NR 46 TC 1 Z9 1 U1 16 U2 29 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1523-7060 EI 1523-7052 J9 ORG LETT JI Org. Lett. PD JUN 17 PY 2016 VL 18 IS 12 BP 2946 EP 2949 DI 10.1021/acs.orglett.6b01293 PG 4 WC Chemistry, Organic SC Chemistry GA DP2FL UT WOS:000378303400040 PM 27267936 ER PT J AU Dombos, AC Fang, DL Spyrou, A Quinn, SJ Simon, A Brown, BA Cooper, K Gehring, AE Liddick, SN Morrissey, DJ Naqvi, F Sumithrarachchi, CS Zegers, RGT AF Dombos, A. C. Fang, D. -L. Spyrou, A. Quinn, S. J. Simon, A. Brown, B. A. Cooper, K. Gehring, A. E. Liddick, S. N. Morrissey, D. J. Naqvi, F. Sumithrarachchi, C. S. Zegers, R. G. T. TI Total absorption spectroscopy of the beta decay of Ga-76 SO PHYSICAL REVIEW C LA English DT Article ID SIMULATION; SEPARATOR; MASS AB The beta decay of Ga-76 was studied using the technique of total absorption spectroscopy for the first time. The experiment was performed at the National Superconducting Cyclotron Laboratory using the Summing NaI(Tl) detector. The extracted beta-decay feeding intensity distribution and Gamow-Teller transition strength distribution are compared to shell-model calculations to help constrain nuclear matrix elements relevant to the neutrinoless double-beta decay of Ge-76. C1 [Dombos, A. C.; Fang, D. -L.; Spyrou, A.; Quinn, S. J.; Simon, A.; Brown, B. A.; Cooper, K.; Gehring, A. E.; Liddick, S. N.; Morrissey, D. J.; Naqvi, F.; Sumithrarachchi, C. S.; Zegers, R. G. T.] Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA. [Dombos, A. C.; Spyrou, A.; Quinn, S. J.; Zegers, R. G. T.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Dombos, A. C.; Fang, D. -L.; Spyrou, A.; Quinn, S. J.; Naqvi, F.; Zegers, R. G. T.] Michigan State Univ, Joint Inst Nucl Astrophys, E Lansing, MI 48824 USA. [Fang, D. -L.] Jilin Univ, Coll Phys, Changchun 130012, Peoples R China. [Simon, A.] Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. [Simon, A.] Univ Notre Dame, Joint Inst Nucl Astrophys, Notre Dame, IN 46556 USA. [Cooper, K.; Liddick, S. N.; Morrissey, D. J.] Michigan State Univ, Dept Chem, E Lansing, MI 48824 USA. [Gehring, A. E.] Los Alamos Natl Lab, Neutron Sci & Technol Grp, Mail Stop H803, Los Alamos, NM 87545 USA. RP Dombos, AC (reprint author), Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA.; Dombos, AC (reprint author), Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA.; Dombos, AC (reprint author), Michigan State Univ, Joint Inst Nucl Astrophys, E Lansing, MI 48824 USA. EM dombos@nscl.msu.edu RI Zegers, Remco/A-6847-2008 FU National Science Foundation [PHY 1102511, PHY 1430152, PHY 1350234, PHY 1404442] FX This work was supported by the National Science Foundation under Grants No. PHY 1102511 (NSCL), No. PHY 1430152 (JINA-CEE), No. PHY 1350234 (CAREER), and No. PHY 1404442. NR 50 TC 0 Z9 0 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD JUN 17 PY 2016 VL 93 IS 6 AR 064317 DI 10.1103/PhysRevC.93.064317 PG 8 WC Physics, Nuclear SC Physics GA DO8RT UT WOS:000378051900003 ER PT J AU Li, Y Yin, ZP Wang, XC Tam, DW Abernathy, DL Podlesnyak, A Zhang, CL Wang, M Xing, LY Jin, CQ Haule, K Kotliar, G Maier, TA Dai, PC AF Li, Yu Yin, Zhiping Wang, Xiancheng Tam, David W. Abernathy, D. L. Podlesnyak, A. Zhang, Chenglin Wang, Meng Xing, Lingyi Jin, Changqing Haule, Kristjan Kotliar, Gabriel Maier, Thomas A. Dai, Pengcheng TI Orbital Selective Spin Excitations and their Impact on Superconductivity of LiFe1-xCoxAs SO PHYSICAL REVIEW LETTERS LA English DT Article ID IRON-BASED SUPERCONDUCTORS; LIFEAS; PNICTIDES; SYMMETRY; DYNAMICS; ORDER AB We use neutron scattering to study spin excitations in single crystals of LiFe0.88Co0.12As, which is located near the boundary of the superconducting phase of LiFe1-xCoxAs and exhibits non-Fermi-liquid behavior indicative of a quantum critical point. By comparing spin excitations of LiFe0.88Co0.12 As with a combined density functional theory and dynamical mean field theory calculation, we conclude that wave-vector correlated low energy spin excitations are mostly from the d(xy) orbitals, while high-energy spin excitations arise from the d(yz) and d(xz) orbitals. Unlike most iron pnictides, the strong orbital selective spin excitations in the LiFeAs family cannot be described by an anisotropic Heisenberg Hamiltonian. While the evolution of low-energy spin excitations of LiFe1-xCoxAs is consistent with the electron-hole Fermi surface nesting conditions for the dxy orbital, the reduced superconductivity in LiFe0.88Co0.12As suggests that Fermi surface nesting conditions for the d(yz) and d(xz) orbitals are also important for superconductivity in iron pnictides. C1 [Li, Yu; Tam, David W.; Zhang, Chenglin; Dai, Pengcheng] Rice Univ, Dept Phys & Astron, Houston, TX 77005 USA. [Yin, Zhiping; Dai, Pengcheng] Beijing Normal Univ, Ctr Adv Quantum Studies, Beijing 100875, Peoples R China. [Yin, Zhiping; Dai, Pengcheng] Beijing Normal Univ, Dept Phys, Beijing 100875, Peoples R China. [Yin, Zhiping; Haule, Kristjan; Kotliar, Gabriel] Rutgers State Univ, Dept Phys, Piscataway, NJ 08854 USA. [Wang, Xiancheng; Xing, Lingyi; Jin, Changqing] Chinese Acad Sci, Inst Phys, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China. [Abernathy, D. L.; Podlesnyak, A.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Wang, Meng] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Jin, Changqing] Collaborat Innovat Ctr Quantum Matter, Beijing, Peoples R China. [Kotliar, Gabriel] Brookhaven Natl Lab, Upton, NY 11973 USA. [Maier, Thomas A.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci & Comp Sci, Oak Ridge, TN 37831 USA. [Maier, Thomas A.] Oak Ridge Natl Lab, Div Math, Oak Ridge, TN 37831 USA. RP Yin, ZP (reprint author), Beijing Normal Univ, Ctr Adv Quantum Studies, Beijing 100875, Peoples R China.; Yin, ZP (reprint author), Beijing Normal Univ, Dept Phys, Beijing 100875, Peoples R China.; Yin, ZP (reprint author), Rutgers State Univ, Dept Phys, Piscataway, NJ 08854 USA. EM yinzhiping@bnu.edu.cn; pdai@rice.edu RI Podlesnyak, Andrey/A-5593-2013; Dai, Pengcheng /C-9171-2012; Abernathy, Douglas/A-3038-2012; Maier, Thomas/F-6759-2012; BL18, ARCS/A-3000-2012 OI Podlesnyak, Andrey/0000-0001-9366-6319; Dai, Pengcheng /0000-0002-6088-3170; Abernathy, Douglas/0000-0002-3533-003X; Maier, Thomas/0000-0002-1424-9996; FU U.S. DOE [BES DE-SC0012311, DE-AC05-00OR22725]; NSF [DMR-1436006, DMR-1308603, DMR-1405303, DMR-1435918]; Robert A. Welch Foundation [C-1839]; Scientific User Facilities Division, BES, U.S. DOE; NSFC; MOST of China FX The neutron scattering work at Rice is supported by the U.S. DOE, BES DE-SC0012311 (P. D.). The computational work at Rice, ORNL, and Rutgers is supported by NSF DMR-1436006 (P. D.), DMR-1308603 (T. M.), DMR-1405303 (K. H.), and DMR-1435918 (Z. P. Y. and G. K.). The materials effort at Rice is also supported by the Robert A. Welch Foundation Grant No. C-1839 (P. D.). The research at SNS was sponsored by the Scientific User Facilities Division, BES, U.S. DOE. The research used resources of the Oak Ridge Leadership Computing Facility at ORNL, which is supported by U.S. DOE under Contract No. DE-AC05-00OR22725. The work at IOP, CAS is supported by NSFC and MOST of China through research projects. NR 55 TC 3 Z9 3 U1 11 U2 33 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUN 17 PY 2016 VL 116 IS 24 AR 247001 DI 10.1103/PhysRevLett.116.247001 PG 6 WC Physics, Multidisciplinary SC Physics GA DO8UK UT WOS:000378059500013 PM 27367401 ER PT J AU Cuevas, DA Edirisinghe, J Henry, CS Overbeek, R O'Connell, TG Edwards, RA AF Cuevas, Daniel A. Edirisinghe, Janaka Henry, Chris S. Overbeek, Ross O'Connell, Taylor G. Edwards, Robert A. TI From DNA to FBA: How to Build Your Own Genome-Scale Metabolic Model SO FRONTIERS IN MICROBIOLOGY LA English DT Article DE metabolic modeling; metabolic reconstruction; in silico modeling; flux-balance analysis; model SEED; genome annotation ID FLUX BALANCE ANALYSIS; ESCHERICHIA-COLI; SYSTEMS BIOLOGY; ANNOTATION; RECONSTRUCTION; CAPABILITIES; INFORMATION; CHALLENGES; NETWORKS; SOFTWARE AB Microbiological studies are increasingly relying on in silico methods to perform exploration and rapid analysis of genomic data, and functional genomics studies are supplemented by the new perspectives that genome-scale metabolic models offer. A mathematical model consisting of a microbe's entire metabolic map can be rapidly determined from whole-genome sequencing and annotating the genomic material encoded in its DNA. Flux-balance analysis (FBA), a linear programming technique that uses metabolic models to predict the phenotypic responses imposed by environmental elements and factors, is the leading method to simulate and manipulate cellular growth in silico. However, the process of creating an accurate model to use in FBA consists of a series of steps involving a multitude of connections between bioinformatics databases, enzyme resources, and metabolic pathways. We present the methodology and procedure to obtain a metabolic model using PyFBA, an extensible Python based open-source software package aimed to provide a platform where functional annotations are used to build metabolic models (http://linsalrob.github.io/PyFBA). Backed by the Model SEED biochemistry database, PyFBA contains methods to reconstruct a microbe's metabolic map, run FBA upon different media conditions, and gap-fill its metabolism. The extensibility of PyFBA facilitates novel techniques in creating accurate genome-scale metabolic models. C1 [Cuevas, Daniel A.; Edwards, Robert A.] San Diego State Univ, Computat Sci Res Ctr, San Diego, CA 92182 USA. [Edirisinghe, Janaka; Henry, Chris S.] Argonne Natl Lab, Div Math & Comp Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. [Overbeek, Ross] Fellowship Interpretat Genomes, Burr Ridge, IL USA. [O'Connell, Taylor G.; Edwards, Robert A.] San Diego State Univ, Biol & Med Informat Res Ctr, San Diego, CA 92182 USA. [Edwards, Robert A.] San Diego State Univ, Dept Comp Sci, San Diego, CA 92182 USA. [Edwards, Robert A.] San Diego State Univ, Dept Biol, San Diego, CA 92182 USA. RP Cuevas, DA (reprint author), San Diego State Univ, Computat Sci Res Ctr, San Diego, CA 92182 USA. EM dcuevas08@gmail.com FU NSF [CNS-1305112, MCB-1330800]; STEM scholarship award - NSF [DUE-1259951] FX This work is supported by NSF grants CNS-1305112 and MCB-1330800 to ER, and by a STEM scholarship award funded by NSF grant DUE-1259951 to Cuevas. NR 58 TC 0 Z9 0 U1 5 U2 13 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-302X J9 FRONT MICROBIOL JI Front. Microbiol. PD JUN 17 PY 2016 VL 7 AR 907 DI 10.3389/fmicb.2016.00907 PG 12 WC Microbiology SC Microbiology GA DO7KA UT WOS:000377960100001 PM 27379044 ER PT J AU Baldini, M Postorino, P Malavasi, L Marini, C Chapman, KW Mao, HK AF Baldini, M. Postorino, P. Malavasi, L. Marini, C. Chapman, K. W. Mao, Ho-kwang TI Pair distribution function analysis: The role of structural degrees of freedom in the high-pressure insulator to metal transition of VO2 SO PHYSICAL REVIEW B LA English DT Article ID VANADIUM DIOXIDE; PHASES AB The evolution of the local structure of VO2 was investigated across the pressure-induced insulator to metal transition (IMT) by means of pair distribution function measurements. The pressure behavior of the V-V and V-O bond lengths have been determined. The data demonstrated that the pressure-driven IMT is not activated by the suppression of the Peierls-type distortion. A clear octahedra symmetrization is observed in the metallic phase, suggesting a link between structural degree of freedom and the metallization process. C1 [Baldini, M.] Argonne Natl Lab, Carnegie Inst Washington, Adv Photon Source, Geophys Lab, Argonne, IL 60439 USA. [Postorino, P.] Univ Roma La Sapienza, Dipartimento Fis, Ple A Moro 4, I-00185 Rome, Italy. [Malavasi, L.] Univ Pavia, Dept Chem, Viale Taramelli 16, I-27100 Pavia, Italy. [Malavasi, L.] INSTM, Viale Taramelli 16, I-27100 Pavia, Italy. [Marini, C.] CELLS ALBA, Carretera BP 1413, Cerdanyola Del Valles 08290, Spain. [Chapman, K. W.] Argonne Natl Lab, Xray Sci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Mao, Ho-kwang] Carnegie Inst Sci, Geophys Lab, 5251 Broad Branch Rd NW, Washington, DC 20015 USA. [Mao, Ho-kwang] Ctr High Pressure Sci & Technol Adv Res, 1690 Cailun Rd, Shanghai 201203, Peoples R China. RP Baldini, M (reprint author), Argonne Natl Lab, Carnegie Inst Washington, Adv Photon Source, Geophys Lab, Argonne, IL 60439 USA. EM mbaldini@carnegiescience.edu RI Malavasi, Lorenzo/P-1966-2016; OI Malavasi, Lorenzo/0000-0003-4724-2376 FU Energy Frontier Research in Extreme Environments Center (EFree), an Energy Frontier Research Center - U.S. Department of Energy, Office of Science [DE-SC0001057] FX This work was supported as part of Energy Frontier Research in Extreme Environments Center (EFree), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science under Award No. DE-SC0001057. NR 29 TC 1 Z9 1 U1 13 U2 37 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUN 17 PY 2016 VL 93 IS 24 AR 245137 DI 10.1103/PhysRevB.93.245137 PG 5 WC Physics, Condensed Matter SC Physics GA DO8RN UT WOS:000378051300003 ER PT J AU Kogan, VG Prozorov, R AF Kogan, V. G. Prozorov, R. TI Interband coupling and nonmagnetic interband scattering in +/- s superconductors SO PHYSICAL REVIEW B LA English DT Article ID OVERLAPPING BANDS; IMPURITIES; TEMPERATURE AB A two-band model with repulsive interband coupling and interband potential scattering is considered to elucidate their effects on material properties. In agreement with previous work, we find that the bands' order parameters Delta 1,2 differ, and the larger is at the band with a smaller normal density of states ( DOS), N-n2 < N-n1. However, the bands' energy gaps, as determined by the energy dependence of the DOS, are equal due to scattering. For each temperature, the gaps become zero at a certain critical interband scattering rate; i.e., for strong enough scattering the model material becomes gapless. In the gapless state, the DOS at band 2 is close to the normal state value, whereas at band 1 it has a V shape with nonzero minimum. When the normal bands DOS are mismatched, N-n1 not equal N-n2, the critical temperature T-c is suppressed even in the absence of interband scattering, T-c(N-n1) has a domelike shape. With increasing interband scattering, the London penetration depth at low temperatures evolves from being exponentially flat to a power law and even to near linear behavior in the gapless state, the latter being easily misinterpreted as caused by order parameter nodes. C1 [Kogan, V. G.; Prozorov, R.] Ames Lab, Ames, IA 50011 USA. [Prozorov, R.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. RP Prozorov, R (reprint author), Ames Lab, Ames, IA 50011 USA.; Prozorov, R (reprint author), Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. EM kogan@ameslab.gov; prozorov@ameslab.gov FU U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Science and Engineering Division; U.S. DOE [DE-AC02-07CH11358] FX Discussions with A. Gurevich, V. Mishra and A. Chubukov are gratefully appreciated. We thank Joerg Schmalian who turned our attention to the question of how Tc changes when approaching critical values of the scattering rate and of DOS n1 (Sec. IVB). This work was supported by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Science and Engineering Division. Ames Laboratory is operated for the U.S. DOE by Iowa State University under contract DE-AC02-07CH11358. NR 38 TC 2 Z9 2 U1 2 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUN 17 PY 2016 VL 93 IS 22 AR 224515 DI 10.1103/PhysRevB.93.224515 PG 11 WC Physics, Condensed Matter SC Physics GA DO8RD UT WOS:000378050200004 ER PT J AU Kitamura, N Hasegawa, H Saito, Y Shinohara, I Yokota, S Nagai, T Pollock, CJ Giles, BL Moore, TE Dorelli, JC Gershman, DJ Avanov, LA Paterson, WR Coffey, VN Chandler, MO Sauvaud, JA Lavraud, B Torbert, RB Russell, CT Strangeway, RJ Burch, JL AF Kitamura, N. Hasegawa, H. Saito, Y. Shinohara, I. Yokota, S. Nagai, T. Pollock, C. J. Giles, B. L. Moore, T. E. Dorelli, J. C. Gershman, D. J. Avanov, L. A. Paterson, W. R. Coffey, V. N. Chandler, M. O. Sauvaud, J. A. Lavraud, B. Torbert, R. B. Russell, C. T. Strangeway, R. J. Burch, J. L. TI Shift of the magnetopause reconnection line to the winter hemisphere under southward IMF conditions: Geotail and MMS observations SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE magnetic reconnection; magnetopause; dipole tilt; MMS mission; Geotail spacecraft ID INTERPLANETARY MAGNETIC-FIELD; DIPOLE TILT; DAYSIDE MAGNETOPAUSE; PLASMA; DEPENDENCE AB At 02:13 UT on 18 November 2015 when the geomagnetic dipole was tilted by -27 degrees, the MMS spacecraft observed southward reconnection jets near the subsolar magnetopause under southward and dawnward interplanetary magnetic field conditions. Based on four-spacecraft estimations of the magnetic field direction near the separatrix and the motion and direction of the current sheet, the location of the reconnection line was estimated to be similar to 1.8 R-E or further northward of MMS. The Geotail spacecraft at GSM Z similar to 1.4 R-E also observed southward reconnection jets at the dawnside magnetopause 30-40min later. The estimated reconnection line location was northward of GSM Z similar to 2 R-E. This crossing occurred when MMS observed purely southward magnetic fields in the magnetosheath. The simultaneous observations are thus consistent with the hypothesis that the dayside magnetopause reconnection line shifts from the subsolar point toward the northern (winter) hemisphere due to the effect of geomagnetic dipole tilt. C1 [Kitamura, N.; Hasegawa, H.; Saito, Y.; Shinohara, I.; Yokota, S.] Japan Aerosp Explorat Agcy, Inst Space & Astronaut Sci, Sagamihara, Kanagawa, Japan. [Nagai, T.] Tokyo Inst Technol, Tokyo, Japan. [Pollock, C. J.; Giles, B. L.; Moore, T. E.; Dorelli, J. C.; Gershman, D. J.; Avanov, L. A.; Paterson, W. R.] NASA, Goddard Space Flight Ctr, Greenbelt, MD USA. [Pollock, C. J.] Denali Sci, Healy, AK USA. [Gershman, D. J.] Oak Ridge Associated Univ, Washington, DC USA. [Coffey, V. N.; Chandler, M. O.] NASA, Marshall Space Flight Ctr, Huntsville, AL USA. [Sauvaud, J. A.; Lavraud, B.] IRAP, Toulouse, France. [Torbert, R. B.] Univ New Hampshire, Ctr Space Sci, Durham, NH 03824 USA. [Russell, C. T.; Strangeway, R. J.] Univ Calif Los Angeles, Inst Geophys & Planetary Phys, Los Angeles, CA 90024 USA. [Burch, J. L.] Southwest Res Inst, San Antonio, TX USA. RP Kitamura, N (reprint author), Japan Aerosp Explorat Agcy, Inst Space & Astronaut Sci, Sagamihara, Kanagawa, Japan. EM kitamura@stp.isas.jaxa.jp RI Hasegawa, Hiroshi/A-1192-2007; NASA MMS, Science Team/J-5393-2013 OI Hasegawa, Hiroshi/0000-0002-1172-021X; NASA MMS, Science Team/0000-0002-9504-5214 FU CNES FX The Geotail data are available from DARTS (https://darts.isas.jaxa.jp/stp/geotail/). Wind data were obtained from CDAweb (http://cdaweb.gsfc.nasa.gov/). We acknowledge Vassilis Angelopoulos for use of ARTEMIS data. We acknowledge Eric Grimes and the developing team of the SPEDAS software for the use. IRAP contribution to MMS was supported by CNES. MMS Level-2 data (FPI version 2.1.0 and FGM version 4.18.0) are available from the MMS Science Data Center (https://lasp.colorado.edu/mms/sdc/public/). NR 38 TC 0 Z9 0 U1 2 U2 3 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD JUN 16 PY 2016 VL 43 IS 11 BP 5581 EP 5588 DI 10.1002/2016GL069095 PG 8 WC Geosciences, Multidisciplinary SC Geology GA DR4DN UT WOS:000379851800006 ER PT J AU Hao, YX Zong, QG Zhou, XZ Fu, SY Rankin, R Yuan, CJ Lui, ATY Spence, HE Blake, JB Baker, DN Reeves, GD AF Hao, Y. X. Zong, Q. -G. Zhou, X. -Z. Fu, S. Y. Rankin, R. Yuan, C. -J. Lui, A. T. Y. Spence, H. E. Blake, J. B. Baker, D. N. Reeves, G. D. TI Electron dropout echoes induced by interplanetary shock: Van Allen Probes observations SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE electron dropout echo; energetic particle; solar wind-magnetospheric coupling; interplanetary shock; magnetopause shadowing; drift shell splitting ID INJECTION BOUNDARY MODEL; ENERGETIC PARTICLE; INNER MAGNETOSPHERE; GEOSYNCHRONOUS ORBIT; GEOMAGNETIC STORMS; FLUX; PROTONS; PLASMA; REGION AB On 23 November 2012, a sudden dropout of the relativistic electron flux was observed after an interplanetary shock arrival. The dropout peaks at approximate to 1 MeV and more than 80% of the electrons disappeared from the drift shell. Van Allen twin Probes observed a sharp electron flux dropout with clear energy dispersion signals. The repeating flux dropout and recovery signatures, or dropout echoes, constitute a new phenomenon referred to as a drifting electron dropout with a limited initial spatial range. The azimuthal range of the dropout is estimated to be on the duskside, from approximate to 1300 to 0100 LT. We conclude that the shock-induced electron dropout is not caused by the magnetopause shadowing. The dropout and consequent echoes suggest that the radial migration of relativistic electrons is induced by the strong dusk-dawn asymmetric interplanetary shock compression on the magnetosphere. C1 [Hao, Y. X.; Zong, Q. -G.; Zhou, X. -Z.; Fu, S. Y.] Peking Univ, Inst Space Phys & Appl Technol, Beijing, Peoples R China. [Rankin, R.] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Yuan, C. -J.] Chinese Acad Sci, Inst Geol & Geophys, Beijing, Peoples R China. [Lui, A. T. Y.] Johns Hopkins Univ, Appl Phys Lab, Laurel, MD USA. [Spence, H. E.] Univ New Hampshire, Dept Phys, Inst Earth Oceans & Space, Durham, NH 03824 USA. [Blake, J. B.] Aerosp Corp, POB 92957, Los Angeles, CA 90009 USA. [Baker, D. N.] Los Alamos Natl Lab, Space & Atmospher Sci Grp, Los Alamos, NM USA. [Reeves, G. D.] Univ Colorado, Lab Atmospher & Space Phys, Boulder, CO 80309 USA. RP Zong, QG (reprint author), Peking Univ, Inst Space Phys & Appl Technol, Beijing, Peoples R China. EM qgzong@pku.edu.cn RI Zhou, Xuzhi/D-1831-2011; OI Zhou, Xuzhi/0000-0003-4953-1761; Reeves, Geoffrey/0000-0002-7985-8098 FU National Natural Science Foundation of China [41421003]; Major Project of Chinese National Programs for Fundamental Research and Development [2012CB825603] FX This work was supported by National Natural Science Foundation of China (41421003 and Major Project of Chinese National Programs for Fundamental Research and Development (2012CB825603). We acknowledge Space Physics Data Facility, Goddard Space Flight Center (http://cdaweb.gsfc.nasa.gov/) for providing all data in this article. Thanks Ying Liu and Jie Ren for helpful discussion. NR 33 TC 1 Z9 1 U1 3 U2 9 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD JUN 16 PY 2016 VL 43 IS 11 BP 5597 EP 5605 DI 10.1002/2016GL069140 PG 9 WC Geosciences, Multidisciplinary SC Geology GA DR4DN UT WOS:000379851800008 ER PT J AU Ripoll, JF Reeves, GD Cunningham, GS Loridan, V Denton, M Santolik, O Kurth, WS Kletzing, CA Turner, DL Henderson, MG Ukhorskiy, AY AF Ripoll, J. -F. Reeves, G. D. Cunningham, G. S. Loridan, V. Denton, M. Santolik, O. Kurth, W. S. Kletzing, C. A. Turner, D. L. Henderson, M. G. Ukhorskiy, A. Y. TI Reproducing the observed energy-dependent structure of Earth's electron radiation belts during storm recovery with an event-specific diffusion model SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE radiation belts; slot region; electron losses; wave particle interactions; hiss waves; electron lifetimes ID VAN ALLEN PROBES; PITCH-ANGLE DIFFUSION; PHASE-SPACE DENSITY; RELATIVISTIC ELECTRONS; ULTRARELATIVISTIC ELECTRONS; PROPAGATION ANALYSIS; GRADUAL DIFFUSION; CHORUS WAVE; OUTER ZONE; PLASMASPHERE AB We present dynamic simulations of energy-dependent losses in the radiation belt slot region and the formation of the two-belt structure for the quiet days after the 1 March storm. The simulations combine radial diffusion with a realistic scattering model, based data-driven spatially and temporally resolved whistler-mode hiss wave observations from the Van Allen Probes satellites. The simulations reproduce Van Allen Probes observations for all energies and L shells (2-6) including (a) the strong energy dependence to the radiation belt dynamics (b) an energy-dependent outer boundary to the inner zone that extends to higher L shells at lower energies and (c) an S-shaped energy-dependent inner boundary to the outer zone that results from the competition between diffusive radial transport and losses. We find that the characteristic energy-dependent structure of the radiation belts and slot region is dynamic and can be formed gradually in similar to 15days, although the S shape can also be reproduced by assuming equilibrium conditions. The highest-energy electrons (E>300keV) of the inner region of the outer belt (L similar to 4-5) also constantly decay, demonstrating that hiss wave scattering affects the outer belt during times of extended plasmasphere. Through these simulations, we explain the full structure in energy and L shell of the belts and the slot formation by hiss scattering during storm recovery. We show the power and complexity of looking dynamically at the effects over all energies and L shells and the need for using data-driven and event-specific conditions. C1 [Ripoll, J. -F.; Loridan, V.] CEA, DAM, DIF, Arpajon, France. [Reeves, G. D.; Cunningham, G. S.; Henderson, M. G.] Los Alamos Natl Lab, Los Alamos, NM USA. [Reeves, G. D.; Cunningham, G. S.; Denton, M.] New Mexico Consortium, Los Alamos, NM USA. [Denton, M.] Space Sci Inst, Boulder, CO USA. [Santolik, O.] Inst Atmospher Phys ASCR, Prague, Czech Republic. [Santolik, O.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Kurth, W. S.; Kletzing, C. A.] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. [Turner, D. L.] Aerosp Corp, Dept Space Sci, El Segundo, CA 90245 USA. [Ukhorskiy, A. Y.] Johns Hopkins Univ, Appl Phys Lab, Laurel, MD USA. RP Ripoll, JF (reprint author), CEA, DAM, DIF, Arpajon, France. EM jean-francois.ripoll@cea.fr RI Santolik, Ondrej/F-7766-2014; Henderson, Michael/A-3948-2011; OI Henderson, Michael/0000-0003-4975-9029; Cunningham, Gregory/0000-0001-8819-4345; Reeves, Geoffrey/0000-0002-7985-8098 FU RBSP-Energetic Particle, Composition, and Thermal Plasma under NASA [NAS5-01072]; JHU/APL under NASA [NAS5-01072, 921647]; Praemium Academiae award; [LH14010]; [LH15304] FX This work was performed under the auspices of an agreement between CEA/DAM and NNSA/DP on cooperation on fundamental science. This work was supported by RBSP-Energetic Particle, Composition, and Thermal Plasma funding under NASA's Prime contract NAS5-01072. The research at University of Iowa was supported by JHU/APL contract 921647 under NASA prime contract NAS5-01072. The authors acknowledge the International Space Sciences Institute (ISSI) and the participants in a 2014 ISSI workshop. O.S. was supported by the LH14010 and LH15304 grants and from the Praemium Academiae award. All Van Allen Probes (RBSP) observations used in this study, along with display and analysis software, are publicly available at the Web site http://www.RBSP-ect.lanl.gov/. For further information or right to access to the computer programs used in this paper, readers can contact the authors. NR 60 TC 5 Z9 5 U1 1 U2 2 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD JUN 16 PY 2016 VL 43 IS 11 BP 5616 EP 5625 DI 10.1002/2016GL068869 PG 10 WC Geosciences, Multidisciplinary SC Geology GA DR4DN UT WOS:000379851800010 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Aben, R Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Agricola, J Aguilar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TPA Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Alkire, SP Allbrooke, BMM Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Piqueras, DA Alviggi, MG Amadio, BT Amako, K Coutinho, A Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, F Anders, G Anders, JK Anderson, KJ Andreazza, A Andrei, V Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Arabidze, G Arai, Y Araque, JP Arce, ATH Arduh, FA Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Arnaez, O Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Asai, S Asbah, N Ashkenazi, A Asman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Augsten, K Aurousseau, M Avolio, G Axen, B Ayoub, MK Azuelos, G Baak, MA Baas, AE Baca, MJ Bacci, C Bachacou, H Bachas, K Backes, M Backhaus, M Bagiacchi, P Bagnaia, P Bai, Y Bain, T Baines, JT Baker, OK Baldin, EM Balek, P Balestri, T Balli, F Balunas, WK Banas, E Banerjee, S Bannoura, AAE Barak, L Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnes, SL Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, P Basalaev, A Bassalat, A Basye, A Bates, RL Batista, SJ Batley, JR 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JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blanco, JE Blazek, T Bloch, I Blocker, C Blum, W Blumenschein, U Blunier, S Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Bock, C Boehler, M Bogaerts, JA Bogavac, D Bogdanchikov, AG Bohm, C Boisvert, V Bold, T Boldea, V Boldyrev, AS Bomben, M Bona, M Boonekamp, M Borisov, A Borissov, G Borroni, S Bortfeldt, J Bortolotto, V Bos, K Boscherini, D Bosman, M Boudreau, J Bouffard, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boutle, SK Boveia, A Boyd, J Boyko, IR Bozic, I Bracinik, J Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Madden, WDB Brendlinger, K Brennan, AJ Brenner, L Brenner, R Bressler, S Bristow, TM Britton, D Britzger, D Brochu, FM Brock, I Brock, R Bronner, J Brooijmans, G Brooks, T Brooks, WK Brosamer, J Brost, E De Renstrom, PAB Bruncko, D Bruneliere, R Bruni, A Bruni, G Bruschi, M Bruscino, N Bryngemark, L Buanes, T Buat, Q Buchholz, P Buckley, AG Buda, SI Budagov, IA Buehrer, F 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F Cerv, M Cervelli, A Cetin, SA Chafaq, A Chakraborty, D Chalupkova, I Chan, YL Chang, P Chapman, JD Charlton, DG Chau, CC Barajas, CAC Cheatham, S Chegwidden, A Chekanov, S Chekulaev, SV Chelkov, GA Chelstowska, MA Chen, C Chen, H Chen, K Chen, L Chen, S Chen, S Chen, X Chen, Y Cheng, HC Cheng, Y Cheplakov, A Cheremushkina, E El Moursli, RC Chernyatin, V Cheu, E Chevalier, L Chiarella, V Chiarelli, G Chiodini, G Chisholm, AS Chislett, RT Chitan, A Chizhov, MV Choi, K Chouridou, S Chow, BKB Christodoulou, V Chromek-Burckhart, D Chudoba, J Chuinard, AJ Chwastowski, JJ Chytka, L Ciapetti, G Ciftci, AK Cinca, D Cindro, V Cioara, IA Ciocio, A Cirotto, F Citron, ZH Ciubancan, M Clark, A Clark, BL Clark, PJ Clarke, RN Clement, C Coadou, Y Cobal, M Coccaro, A Cochran, J Coffey, L Cogan, JG Colasurdo, L Cole, B Cole, S Colijn, AP Collot, J Colombo, T Compostella, G Muino, PC Coniavitis, E Connell, SH Connelly, IA Consorti, V Constantinescu, S Conta, C Conti, G Conventi, F Cooke, M Cooper, BD 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Delitzsch, CM Deliyergiyev, M Dell'Acqua, A Dell'Asta, L Dell'Orso, M Della Pietra, M della Volpe, D Delmastro, M Delsart, PA Deluca, C DeMarco, DA Demers, S Demichev, M Demilly, A Denisov, SP Derendarz, D Derkaoui, JE Derue, F Dervan, P Desch, K Deterre, C Dette, K Deviveiros, PO Dewhurst, A Dhaliwal, S Di Ciaccio, A Di Ciaccio, L Di Domenico, A Di Donato, C Di Girolamo, A Di Girolamo, B Di Mattia, A Di Micco, B Di Nardo, R Di Simone, A Di Sipio, R Di Valentino, D Diaconu, C Diamond, M Dias, FA Diaz, MA Diehl, EB Dietrich, J Diglio, S Dimitrievska, A Dingfelder, J Dita, P Dita, S Dittus, F Djama, F Djobava, T Djuvsland, JI do Vale, MAB Dobos, D Dobre, M Doglioni, C Dohmae, T Dolejsi, J Dolezal, Z Dolgoshein, BA Donadelli, M Donati, S Dondero, P Donini, J Dopke, J Doria, A Dova, MT Doyle, AT Drechsler, E Dris, M Dubreuil, E Duchovni, E Duckeck, G Doyle, AT Drechsler, E Dris, M Dubreuil, E Duchovni, E Duckeck, G Ducu, OA Duda, D Dudarev, A Duflot, L Duguid, L Duhrssen, M Dunford, M 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CA ATLAS Collaboration TI Identification of high transverse momentum top quarks in pp collisions at root s=8 TeV with the ATLAS detector SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron scattering (experiments) ID PAIR PRODUCTION; PARTON DISTRIBUTIONS; HADRON COLLIDERS; RESUMMATION; LHC AB This paper presents studies of the performance of several jet-substructure techniques, which are used to identify hadronically decaying top quarks with high transverse momentum contained in large-radius jets. The efficiency of identifying top quarks is measured using a sample of top-quark pairs and the rate of wrongly identifying jets from other quarks or gluons as top quarks is measured using multijet events collected with the ATLAS experiment in 20.3 fb(-1) of 8TeV proton-proton collisions at the Large Hadron Collider. Predictions from Monte Carlo simulations are found to provide an accurate description of the performance. The techniques are compared in terms of signal efficiency and background rejection using simulations, covering a larger range in jet transverse momenta than accessible in the dataset. Additionally, a novel technique is developed that is optimized to reconstruct top quarks in events with many jets. C1 [Jackson, P.; Lee, L.; Petridis, A.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Edson, W.; Ernst, J.; Fischer, A.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Butt, A. I.; Czodrowski, P.; Dassoulas, J.; Gingrich, D. M.; Jabbar, S.; Karamaoun, A.; Moore, R. W.; Pinfold, J. L.; Saddique, A.; Vaque, F. Vives] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Ciftci, A. K.; Yildiz, H. Duran] Ankara Univ, Dept Phys, Ankara, Turkey. [Kuday, S.] Istanbul Aydin Univ, Istanbul, Turkey. [Sultansoy, S.] TOBB Univ Econ & Technol, Div Phys, Ankara, Turkey. 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O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duhrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Feng, E. J.; Perez, S. Fernandez; Francis, D.; Froidevaux, D.; Gadatsch, S.; Gillberg, D.; Glatzer, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hawkings, R. J.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Huhtinen, M.; Iengo, P.; Jaekel, M. R.; Jakobsen, S.; Jenni, P.; Klioutchnikova, T.; Krasznahorkay, A.; Lapoire, C.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Marzin, A.; Milic, A.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Ohman, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Ritsch, E.; Roe, S.; Ruiz-Martinez, A.; Ruthmann, N.; Salzburger, A.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sforza, F.; Sfyrla, A.; Sanchez, C. A. Solans; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van Woerden, M. C.; Vandelli, W.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Toro, R. Camacho; Cheng, Y.; Dandoy, J. R.; Facini, G.; Fiascaris, M.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Kim, Y. K.; Krizka, K.; Li, H. L.; Merritt, F. S.; Miller, D. W.; Narayan, R.; Okawa, H.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Vukotic, I.; Webster, J. S.; Wu, M.] Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Blunier, S.; Carquin, E.; Diaz, M. A.; Ochoa-Ricoux, J. P.; Vogel, M.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; Salazar Loyola, J. E.; Tapia Araya, S.; White, R.] Univ Tecn Feder Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Gao, J.; Jin, S.; Lou, X.; Ouyang, Q.; Peng, C.; Ren, H.; Shan, L. Y.; Sun, X.; Xu, D.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Ge, P.; Guo, Y.; Han, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, M.; Liu, Y.; Peng, H.; Song, H. Y.; Zhang, G.; Zhang, R.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Li, Y.; Zhang, H.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Liu, B.; Ma, L. L.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Bret, M. Cano; Guo, J.; Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Shanghai Key Lab Particle Phys & Cosmol, Dept Phys & Astron, Shanghai, Peoples R China. [Bret, M. Cano; Guo, J.; Li, L.; Yang, H.] PKU CHEP, Beijing, Peoples R China. [Chen, X.; Zhou, N.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Clermont Univ, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] CNRS, IN2P3, Clermont Ferrand, France. [Alkire, S. P.; Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Carbone, R. M.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Nikiforou, N.; Ochoa, I.; Parsons, J. A.; Smith, M. N. K.; Smith, R. W.; Thompson, E. N.; Tuts, P. M.; Wang, T.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Besjes, G. J.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] INFN, Grp Collegato Cosenza, Lab Nazl Frascati, Arcavacata Di Rende, Italy. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; De Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Knapik, J.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] Southern Methodist Univ, Dept Phys, Dallas, TX USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Hamburg, Germany. [Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Cakir, O.; Dette, K.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bjergaard, D. M.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; Molander, S.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Giromini, P.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] INFN, Lab Nazl Frascati, Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Burgard, C. D.; Buescher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Landgraf, U.; Luedtke, C.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Sammel, D.; Schillo, C.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Ta, D.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; Von Radziewski, H.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, Freiburg, Germany. [Ancu, L. S.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Calace, N.; Clark, A.; Coccaro, A.; Delitzsch, C. M.; della Volpe, D.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Nessi, M.; Paolozzi, L.; Picazio, A.; Ristic, B.; Schramm, S.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] INFN, Sez Genova, Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Durglishvili, A.; Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Phys Inst 2, Giessen, Germany. [Bates, R. L.; Boutle, S. K.; Madden, W. D. Breaden; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; de Lima, D. E. Ferreira; Gul, U.; Knue, A.; Morton, A.; Mullen, P.; O'Shea, V.; Barrera, C. Oropeza; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; Denis, R. D. St.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Agricola, J.; Bindi, M.; Blumenschein, U.; Brandt, G.; Drechsler, E.; George, M.; Graber, L.; Grosse-Knetter, J.; Janus, M.; Kareem, M. J.; Kawamura, G.; Lai, S.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Phys Inst 2, Gottingen, Germany. [Albrand, S.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, Lab Phys Subatom & Cosmol, CNRS, IN2P3, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Catastini, P.; Clark, B. L.; Franklin, M.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Tuna, A. N.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Theenhausen, H. Meyer Zu; Villar, D. I. Narrias; Sahinsoy, M.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Starovoitov, P.; Suchek, S.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Kolb, M.; Lisovyi, M.; Schaetzel, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Phys Inst, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Chan, Y. L.; Castillo, L. R. Flores; Lu, H.; Salvucci, A.; Tsui, K. M.] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R.; Jussel, P.; Kneringer, E.; Lukas, W.; Usanova, A.; Vigne, R.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Argyropoulos, S.; Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Krumnack, N.; Pluth, D.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Dubna, Russia. [Amako, K.; Aoki, M.; Hanagaki, K.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, S.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Yamada, M.; Yamamoto, A.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Kido, S.; Kishimoto, T.; Kurashige, H.; Maeda, J.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo, Japan. [Ishino, M.; Kunigo, T.; Monden, R.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka, Japan. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] INFN, Sez Lecce, Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Univ Ljubljana, Ljubljana, Slovenia. [Bevan, A. J.; Bona, M.; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Sowden, B. C.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Ortiz, N. G. Gutierrez; Hesketh, G. G.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.; Yap, Y. C.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.; Yap, Y. C.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.; Yap, Y. C.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Lytken, E.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fysiska Inst, Lund, Sweden. [Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor, C-15, Madrid, Spain. [Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Cuth, J.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Koepke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schott, M.; Schuh, N.; Simioni, E.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Keoshkerian, H.; Li, X.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Pin, A. W. J.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Schwanenberger, C.; Schweiger, H.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Zhang, R.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Zhang, R.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Taylor, P. T. E.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Guan, L.; Guo, Y.; Hu, X.; Levin, D.; Liu, H.; Lu, N.; Marley, D. E.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Thun, R. P.; Wilson, A.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Burckhart, H.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Tollefson, K.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazza, S. M.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Stabile, A.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] INFN, Sez Milano, Milan, Italy. [Andreazza, A.; Carminati, L.; Fanti, M.; Mazza, S. M.; Perini, L.; Pizio, C.; Ragusa, F.; Shojaii, S.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Russian Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] ITEP, Moscow, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Tikhomirov, V. O.; Timoshenko, S.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Elmsheuser, J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Giuliani, C.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Manfredini, A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Spettel, F.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, Munich, Germany. [Fusayasu, T.; Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Horii, Y.; Kawade, K.; Morvaj, L.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi, Japan. [Horii, Y.; Kawade, K.; Morvaj, L.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Cirotto, F.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] INFN, Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Cirotto, F.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Napoli, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Caron, S.; Colasurdo, L.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Konig, A. C.; Nektarijevic, S.; Strubig, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Andari, N.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Saha, P.; Yurkewicz, A.] Northern Illinois Univ, Dept Phys, De Kalb, IL USA. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA. [Beacham, J. B.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Nagarkar, A.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; De Benedetti, A.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Rifki, O.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Etzion, E.; Haley, J.; Jamin, D. O.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, Olomouc, Czech Republic. [Abreu, R.; Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris Saclay, CNRS IN2P3, Univ Paris 11, LAL, Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Oide, H.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pickering, M. A.; Ryder, N. C.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Introzzi, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] INFN, Sez Pavia, Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Introzzi, G.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, Pavia, Italy. [Balunas, W. K.; Brendlinger, K.; Fletcher, R. R. M.; Haney, B.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Miguens, J. Machado; Meyer, C.; Mistry, K. P.; Reichert, J.; Stahlman, J.; Thomson, E.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Fiolhais, M. C. N.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] BP Konstantinov Petersburg Nucl Phys Inst, Kurchatov Inst, Natl Res Ctr, St Petersburg, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] INFN, Sez Pisa, Pisa, Italy. [Annovi, A.; Bertolucci, F.; Biesuz, N. V.; Chiarelli, G.; Dell'Orso, M.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Escobar, C.; Hong, T. M.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; De Sousa, M. J. Da Cunha Sargedas; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Santos, H.; Saraiva, J. G.; Silva, J.; Tavares Delgado, A.; Veloso, F.; Wolters, H.] LIP, Lab Instrument & Fis Expt Particulas, Lisbon, Portugal. [Amorim, A.; Conde Muino, P.; De Sousa, M. J. Da Cunha Sargedas; Galhardo, B.; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Saraiva, J. G.; Tavares Delgado, A.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, P.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Ryzhov, A.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] State Res Ctr Inst High Energy Phys Protvino, Nrc Ki, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot, Oxon, England. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Di Donato, C.; Falciano, S.; Gauzzi, P.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] INFN, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; Di Domenico, A.; Di Donato, C.; Gauzzi, P.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Sapienza Univ Roma, Dipartimento Fis, Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Salamon, A.; Santonico, R.] INFN, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.] INFN, Sez Roma Tre, Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.; Ouchrif, M.; Tayalati, Y.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA Marrakech, Marrakech, Morocco. [Derkaoui, J. E.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed 5, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Kivernyk, O.; Kozanecki, W.; Kukla, R.; Con, E. Lan; Laporte, J. F.; Maiani, C.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] CEA Saclay Commissariat & Energie Atom & Energie, DSM IRFU Inst Recherches Lois Fondament Univ, Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Fedorko, W.; Grabas, H. M. X.; Grillo, A. A.; Hance, M.; Kuhl, A.; La Rosa, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Alpigiani, C.; Blackburn, D.; Goussiou, A. G.; Hsu, S. -C.; Johnson, W. J.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Pastor, E. Torro; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hamity, G. N.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ghasemi, S.; Ibragimov, I.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Temple, D.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Ilic, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Moss, J.; Mount, R.; Nachman, B. P.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Strauss, E.; Su, D.; Swiatlowski, M.; Tompkins, L.; Wittgen, M.; Young, C.; Zeng, Q.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Plazak, L.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Annovi, A.; Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnuclear Phys, Kosice, Slovakia. [Castaneda-Miranda, E.; Hamilton, A.; Lee, C. A.; Meehan, S.; Yacoob, S.] Univ Cape Town, Dept Phys, Cape Town, South Africa. [Aurousseau, M.; Connell, S. H.; Govender, N.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Hsu, C.; Kar, D.; March, L.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Stockholm Univ, Dept Phys, Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Sidebo, P. E.; Strandberg, J.] Royal Inst Technol, Dept Phys, Stockholm, Sweden. [Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Montalbano, A.; Puldon, D.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Allbrooke, B. M. M.; Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Morley, A. K.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Wang, J.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW, Australia. [Abdallah, J.; Hou, S.; Hsu, P. J.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Song, H. Y.; Teng, P. K.; Wang, C.; Wang, S. M.; Yang, Y.] Acad Sin, Inst Phys, Taipei, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia, A.; Gozani, E.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Blazek, T.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgiou, K.; Hernandez, D. Paredes; Petridou, C.; Sampsonidis, D.; Tsionou, D.] Aristotle Univ Thessaloniki, Dept Phys, Thessaloniki, Greece. [Aloisio, A.; Asai, S.; Chen, S.; Dohmae, T.; Hanawa, K.; Kanaya, N.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Mashimo, T.; Masubuchi, T.; Mori, T.; Morinaga, M.; Nakamura, T.; Sakamoto, H.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Pettersson, N. E.; Todome, K.; Yamaguchi, D.] Tokyo Inst Technol, Dept Phys, Tokyo, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Veloce, L. M.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Gingrich, D. M.; Jovicevic, J.; Koutsman, A.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, Vancouver, BC, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON, Canada. [Hara, K.; Hayashi, T.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okamura, W.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Hara, K.; Hayashi, T.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okamura, W.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Ctr Integrated Res Fundamental Sci & Engn, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Corso-Radu, A.; Frate, M.; Gerbaudo, D.; Guest, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Barisonzi, M.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Quayle, W. B.; Serkin, L.; Shaw, K.; Soualah, R.; Truong, L.] INFN, Grp Collegato Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; Barisonzi, M.; Cobal, M.; Quayle, W. B.; Serkin, L.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Soualah, R.; Truong, L.] Univ Udine, Dipartimento Chim Fis & Ambiente, Udine, Italy. [Atkinson, M.; Basye, A.; Armadans, R. Caminal; Cavaliere, V.; Chang, P.; Errede, S.; Lie, K.; Liss, T. M.; Liu, L.; Long, J. D.; Neubauer, M. S.; Rybar, M.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, 1110 W Green St, Urbana, IL 61801 USA. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Lopez, S. Pedraza; Perez Garcia-Estan, M. T.; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Lopez, S. Pedraza; Perez Garcia-Estan, M. T.; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Lopez, S. Pedraza; Perez Garcia-Estan, M. T.; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Lopez, S. Pedraza; Perez Garcia-Estan, M. T.; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Ferrer, J. A. Valls; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Lopez, S. Pedraza; Perez Garcia-Estan, M. T.; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Ferrer, J. A. Valls; Vos, M.] CSIC, Valencia, Spain. [Danninger, M.; Gay, C.; Gecse, Z.; Gignac, M.; Henkelmann, S.; King, S. B.; Lister, A.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; Berghaus, F.; David, C.; Elliot, A. A.; Fincke-Keeler, M.; Hamano, K.; Hill, E.; Keeler, R.; Kowalewski, R.; Kuwertz, E. S.; Kwan, T.; LeBlanc, M.; Lefebvre, M.; Marino, C. P.; McPherson, R. A.; Pearce, J.; Sobie, R.; Trovatelli, M.; Venturi, M.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Beckingham, M.; Farrington, S. M.; Harrison, P. F.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.; Spangenberg, M.] Univ Warwick, Dept Phys, Coventry, W Midlands, England. [Iizawa, T.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Bressler, S.; Citron, Z. H.; Duchovni, E.; Gross, E.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Pitt, M.; Roth, I.; Schaarschmidt, J.; Smakhtin, V.] Weizmann Inst Sci, Dept Particle Phys, Rehovot, Israel. [Banerjee, Sw.; Hard, A. S.; Heng, Y.; Ji, H.; Ju, X.; Kaplan, L. S.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, 1150 Univ Ave, Madison, WI 53706 USA. [Kuger, F.; Redelbach, A.; Schreyer, M.; Sidiropoulou, O.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Univ Wurzburg, Fak Phys & Astron, Wurzburg, Germany. [Bannoura, A. A. E.; Braun, H. M.; Cornelissen, T.; Ellinghaus, F.; Ernis, G.; Fischer, J.; Flick, T.; Gabizon, O.; Hamacher, K.; Harenberg, T.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Kohlmann, S.; Maettig, P.; Neumann, M.; Pataraia, S.; Riegel, C. J.; Sandhoff, M.; Tepel, F.; Wagner, W.; Zeitnitz, C.] Berg Univ Wuppertal, Fachgrp Phys, Fak Math Naturwissensch, Wuppertal, Germany. [Baker, O. K.; Cummings, J.; Demers, S.; Garberson, F.; Henrichs, A.; Ideal, E.; Lagouri, T.; Leister, A. G.; Loginov, A.; Thomsen, L. A.; Tipton, P.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan, Armenia. [Rahal, G.] Ctr Calcul Inst Natl Phys Nucl & Phys Particules, IN2P3, Villeurbanne, France. Kings Coll London, Dept Phys, London, England. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk, Russia. [Bawa, H. S.; Gao, Y. S.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beck, H. P.] Univ Fribourg, Dept Phys, Fribourg, Switzerland. [Casado, M. P.] Univ Autonoma Barcelona, Dept Fis, Barcelona, Spain. [Castro, N. F.] Univ Porto, Fac Ciencias, Dept Fis & Astron, Rua Campo Alegre 823, P-4100 Oporto, Portugal. [Chelkov, G. A.] Tomsk State Univ, Tomsk, Russia. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Corriveau, F.; McPherson, R. A.; Robertson, S. H.; Sobie, R.; Teuscher, R. J.] IPP, Waterloo, ON, Canada. [Fedin, O. L.] St Petersburg State Polytech Univ, Dept Phys, St Petersburg, Russia. [Grinstein, S.; Juste Rozas, A.; Martinez, M.] ICREA, Barcelona, Spain. [Hsu, P. J.] Natl Tsing Hua Univ, Dept Phys, Hsinchu 30013, Taiwan. [Ilchenko, Y.; Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Jejelava, J.] Ilia State Univ, Inst Theoret Phys, Tbilisi, Rep of Georgia. [Khubua, J.] GTU, Tbilisi, Rep of Georgia. [Kono, T.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Leisos, A.] Hellen Open Univ, Patras, Greece. [Lin, S. C.] Acad Sin, Inst Phys, Acad Sinica Grid Comp, Taipei, Taiwan. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys, Dolgoprudnyi, Russia. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Technol State Univ, Dolgoprudnyi, Russia. [Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ South Carolina, Dept Phys & Astron, Columbia, SC USA. [Shi, L.; Soh, D. A.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou, Guangdong, Peoples R China. [Shiyakova, M.] Bulgarian Acad Sci, INRNE, Sofia, Bulgaria. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Spannowsky, M.] Univ Durham, IPPP, Durham, England. [Tompkins, L.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Vest, A.] Flensburg Univ Appl Sci, Flensburg, Germany. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur, Malaysia. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France. RI Chekulaev, Sergey/O-1145-2015; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Carli, Ina/C-2189-2017; Guo, Jun/O-5202-2015; Peleganchuk, Sergey/J-6722-2014; Yang, Haijun/O-1055-2015; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Kuday, Sinan/C-8528-2014; Garcia, Jose /H-6339-2015; Gavrilenko, Igor/M-8260-2015; Owen, Mark/Q-8268-2016; Di Domenico, Antonio/G-6301-2011; Shulga, Evgeny/R-1759-2016; Gauzzi, Paolo/D-2615-2009; Maleev, Victor/R-4140-2016; Mitsou, Vasiliki/D-1967-2009; Camarri, Paolo/M-7979-2015; Mindur, Bartosz/A-2253-2017; Mashinistov, Ruslan/M-8356-2015; Gutierrez, Phillip/C-1161-2011; Fabbri, Laura/H-3442-2012; Kantserov, Vadim/M-9761-2015; Conde Muino, Patricia/F-7696-2011; Grinstein, Sebastian/N-3988-2014; Zhukov, Konstantin/M-6027-2015; Stabile, Alberto/L-3419-2016; Warburton, Andreas/N-8028-2013; Boyko, Igor/J-3659-2013; Villa, Mauro/C-9883-2009; Coccaro, Andrea/P-5261-2016; Brooks, William/C-8636-2013; Staroba, Pavel/G-8850-2014; Kukla, Romain/P-9760-2016; Goncalo, Ricardo/M-3153-2016; Smirnova, Oxana/A-4401-2013; Di Nardo, Roberto/J-4993-2012; Tikhomirov, Vladimir/M-6194-2015; Maneira, Jose/D-8486-2011; Gladilin, Leonid/B-5226-2011; Livan, Michele/D-7531-2012; Carvalho, Joao/M-4060-2013; messina, andrea/C-2753-2013; Prokoshin, Fedor/E-2795-2012; Doyle, Anthony/C-5889-2009; Ventura, Andrea/A-9544-2015 OI Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Carli, Ina/0000-0002-0411-1141; Guo, Jun/0000-0001-8125-9433; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Kuday, Sinan/0000-0002-0116-5494; Owen, Mark/0000-0001-6820-0488; Di Domenico, Antonio/0000-0001-8078-2759; Shulga, Evgeny/0000-0001-5099-7644; Gauzzi, Paolo/0000-0003-4841-5822; Mitsou, Vasiliki/0000-0002-1533-8886; Camarri, Paolo/0000-0002-5732-5645; Mindur, Bartosz/0000-0002-5511-2611; Mashinistov, Ruslan/0000-0001-7925-4676; Fabbri, Laura/0000-0002-4002-8353; Kantserov, Vadim/0000-0001-8255-416X; Conde Muino, Patricia/0000-0002-9187-7478; Grinstein, Sebastian/0000-0002-6460-8694; Stabile, Alberto/0000-0002-6868-8329; Warburton, Andreas/0000-0002-2298-7315; Boyko, Igor/0000-0002-3355-4662; Villa, Mauro/0000-0002-9181-8048; Coccaro, Andrea/0000-0003-2368-4559; Brooks, William/0000-0001-6161-3570; Kukla, Romain/0000-0002-1140-2465; Goncalo, Ricardo/0000-0002-3826-3442; Smirnova, Oxana/0000-0003-2517-531X; Tikhomirov, Vladimir/0000-0002-9634-0581; Maneira, Jose/0000-0002-3222-2738; Gladilin, Leonid/0000-0001-9422-8636; Livan, Michele/0000-0002-5877-0062; Carvalho, Joao/0000-0002-3015-7821; Prokoshin, Fedor/0000-0001-6389-5399; Doyle, Anthony/0000-0001-6322-6195; Ventura, Andrea/0000-0002-3368-3413 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; HGF, Germany; MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SERI, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE, United States of America; NSF, United States of America; BCKDF, Canada; Canada Council, Canada; CANARIE, Canada; CRC, Canada; Compute Canada, Canada; FQRNT, Canada; Ontario Innovation Trust, Canada; EPLANET, European Union; ERC, European Union; FP7, European Union; Horizon, European Union; Marie Sklodowska-Curie Actions, European Union; Investissement d'Avenir Labex, France; Investissement d'Avenir Idex, France; ANR, France; Region Auvergne, France; Fondation Partager le Savoir, France; DFG, Germany; AvH Foundation, Germany; Herakleitos programme - EU-ESF; Thales programme - EU-ESF; Aristeia programme - EU-ESF; Greek NSRF; BSF, Israel; GIF, Israel; Minerva, Israel; BRF, Norway; Generalitat de Catalunya, Generalitat Valenciana, Spain; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF and DNSRC, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, HGF, and MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW and NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SERI, SNSF and Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE and NSF, United States of America. In addition, individual groups and members have received support from BCKDF, the Canada Council, CANARIE, CRC, Compute Canada, FQRNT, and the Ontario Innovation Trust, Canada; EPLANET, ERC, FP7, Horizon 2020 and Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR, Region Auvergne and Fondation Partager le Savoir, France; DFG and AvH Foundation, Germany; Herakleitos, Thales and Aristeia programmes co-financed by EU-ESF and the Greek NSRF; BSF, GIF and Minerva, Israel; BRF, Norway; Generalitat de Catalunya, Generalitat Valenciana, Spain; the Royal Society and Leverhulme Trust, United Kingdom. NR 95 TC 2 Z9 2 U1 22 U2 49 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JUN 16 PY 2016 IS 6 AR 093 DI 10.1007/JHEP06(2016)093 PG 81 WC Physics, Particles & Fields SC Physics GA DQ4MF UT WOS:000379177300001 ER PT J AU Herring, CD Kenealy, WR Shaw, AJ Covalla, SF Olson, DG Zhang, JY Sillers, WR Tsakraklides, V Bardsley, JS Rogers, SR Thorne, PG Johnson, JP Foster, A Shikhare, ID Klingeman, DM Brown, SD Davison, BH Lynd, LR Hogsett, DA AF Herring, Christopher D. Kenealy, William R. Shaw, A. Joe Covalla, Sean F. Olson, Daniel G. Zhang, Jiayi Sillers, W. Ryan Tsakraklides, Vasiliki Bardsley, John S. Rogers, Stephen R. Thorne, Philip G. Johnson, Jessica P. Foster, Abigail Shikhare, Indraneel D. Klingeman, Dawn M. Brown, Steven D. Davison, Brian H. Lynd, Lee R. Hogsett, David A. TI Strain and bioprocess improvement of a thermophilic anaerobe for the production of ethanol from wood SO BIOTECHNOLOGY FOR BIOFUELS LA English DT Article DE Cellulosic ethanol; Consolidated bioprocessing; Organism development; Metabolic engineering; Bioprocess development; Thermophilic bacteria ID THERMOANAEROBACTERIUM-SACCHAROLYTICUM; ACETOBUTYLICUM; EXPRESSION; PHYSIOLOGY; TOLERANCE; GENES; TOOL AB Background: The thermophilic, anaerobic bacterium Thermoanaerobacterium saccharolyticum digests hemicellulose and utilizes the major sugars present in biomass. It was previously engineered to produce ethanol at yields equivalent to yeast. While saccharolytic anaerobes have been long studied as potential biomass-fermenting organisms, development efforts for commercial ethanol production have not been reported. Results: Here, we describe the highest ethanol titers achieved from T. saccharolyticum during a 4-year project to develop it for industrial production of ethanol from pre-treated hardwood at 51-55 degrees C. We describe organism and bioprocess development efforts undertaken to improve ethanol production. The final strain M2886 was generated by removing genes for exopolysaccharide synthesis, the regulator perR, and re-introduction of phosphotransacetylase and acetate kinase into the methyglyoxal synthase gene. It was also subject to multiple rounds of adaptation and selection, resulting in mutations later identified by resequencing. The highest ethanol titer achieved was 70 g/L in batch culture with a mixture of cellobiose and maltodextrin. In a "mock hydrolysate" Simultaneous Saccharification and Fermentation (SSF) with Sigmacell-20, glucose, xylose, and acetic acid, an ethanol titer of 61 g/L was achieved, at 92 % of theoretical yield. Fungal cellulases were rapidly inactivated under these conditions and had to be supplemented with cellulosomes from C. thermocellum. Ethanol titers of 31 g/L were reached in a 100 L SSF of pre-treated hardwood and 26 g/L in a fermentation of a hardwood hemicellulose extract. Conclusions: This study demonstrates that thermophilic anaerobes are capable of producing ethanol at high yield and at titers greater than 60 g/L from purified substrates, but additional work is needed to produce the same ethanol titers from pre-treated hardwood. C1 [Herring, Christopher D.; Kenealy, William R.; Shaw, A. Joe; Covalla, Sean F.; Zhang, Jiayi; Sillers, W. Ryan; Tsakraklides, Vasiliki; Bardsley, John S.; Rogers, Stephen R.; Thorne, Philip G.; Johnson, Jessica P.; Foster, Abigail; Shikhare, Indraneel D.; Lynd, Lee R.; Hogsett, David A.] Mascoma Corp, 67 Etna Rd, Lebanon, NH 03766 USA. [Herring, Christopher D.; Olson, Daniel G.; Lynd, Lee R.] Dartmouth Coll, Thayer Sch Engn, 14 Engn Dr, Hanover, NH 03755 USA. [Kenealy, William R.] Verdezyne, Carlsbad, CA USA. [Shaw, A. Joe; Tsakraklides, Vasiliki] Novogy Inc, Cambridge, MA 02138 USA. [Olson, Daniel G.; Klingeman, Dawn M.; Brown, Steven D.; Davison, Brian H.; Lynd, Lee R.] Bioenergy Sci Ctr, Oak Ridge, TN USA. [Zhang, Jiayi] Genzyme, Cambridge, MA USA. [Sillers, W. Ryan] Myriant Corp, Quincy, MA USA. [Shikhare, Indraneel D.] Nalco Champ, Houston, TX USA. [Klingeman, Dawn M.; Brown, Steven D.; Davison, Brian H.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN USA. [Hogsett, David A.] Novozymes Inc, Davis, CA USA. RP Herring, CD (reprint author), Mascoma Corp, 67 Etna Rd, Lebanon, NH 03766 USA.; Herring, CD (reprint author), Dartmouth Coll, Thayer Sch Engn, 14 Engn Dr, Hanover, NH 03755 USA. EM chrisherringfish@gmail.com RI Klingeman, Dawn/B-9415-2012 OI Klingeman, Dawn/0000-0002-4307-2560 FU Mascoma Corporation; Department of Energy (DOE) [E-FC36-07G017057]; BioEnergy Science Center, a US DOE Bioenergy Research Center - Office of Biological and Environmental Research in the DOE Office of Science; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; DOE [DE-AC05-00OR22725]; Department of Energy; agency of the US Government FX This work was supported by Mascoma Corporation and the Department of Energy (DOE) under Award Number DE-FC36-07G017057. Manuscript preparation was supported in part by the BioEnergy Science Center, a US DOE Bioenergy Research Center supported by the Office of Biological and Environmental Research in the DOE Office of Science. The work conducted by the U.S. DOE Joint Genome Institute, a DOE Office of Science User Facility, is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. ORNL is managed by UT-Battelle, LLC, Oak Ridge, TN, USA, for the DOE under contract DE-AC05-00OR22725. United States Government retains and the publisher, by accepting the article for publication, acknowledges that the US Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for US Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE-Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). Disclaimer "This report was prepared as an account of work sponsored by an agency of the US Government. Neither the US Government nor any agency thereof, nor any of their employees, makes any warranty, express or implied, or assumes any legal liability or responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would not infringe privately owned rights. Reference herein to any specific commercial product, process, or service by trade name, trademark, manufacturer, or otherwise does not necessarily constitute or imply its endorsement, recommendation, or favoring by the US Government or any agency thereof. The views and opinions of authors expressed herein do not necessarily state or reflect those of the US Government or any agency thereof." NR 25 TC 3 Z9 3 U1 8 U2 16 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1754-6834 J9 BIOTECHNOL BIOFUELS JI Biotechnol. Biofuels PD JUN 16 PY 2016 VL 9 AR 125 DI 10.1186/s13068-016-0536-8 PG 16 WC Biotechnology & Applied Microbiology; Energy & Fuels SC Biotechnology & Applied Microbiology; Energy & Fuels GA DQ0ED UT WOS:000378870300001 PM 27313661 ER PT J AU Kassem, M Sokolov, A Cuisset, A Usuki, T Khaoulani, S Masselin, P Le Coq, D Neuefeind, JC Feygenson, M Hannon, AC Benmore, CJ Bychkov, E AF Kassem, M. Sokolov, A. Cuisset, A. Usuki, T. Khaoulani, S. Masselin, P. Le Coq, D. Neuefeind, J. C. Feygenson, M. Hannon, A. C. Benmore, C. J. Bychkov, E. TI Mercury Sulfide Dimorphism in Thioarsenate Glasses SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID REVERSE-MONTE-CARLO; NEUTRON-DIFFRACTION; X-RAY; AMORPHOUS SOLIDS; MATERIALS DIFFRACTOMETER; RAMAN-SPECTROSCOPY; OPTICAL-PROPERTIES; PHASE-TRANSITIONS; LIQUID; SPACE AB Crystalline mercury sulfide exists in two drastically different polymorphic forms in different domains of the P,T-diagram: red chain-like insulator alpha-HgS, stable below 344 degrees C, and black tetrahedral narrow-band semiconductor beta-HgS, stable at higher temperatures. Using pulsed neutron and high-energy X-ray diffraction, we show that these two mercury bonding patterns are present simultaneously in mercury thioarsenate glasses HgS As2S3. The population and interconnectivity of chain-like and tetrahedral dimorphous forms determine both the structural features and fundamental glass properties (thermal, electronic, etc.). DFT simulations of mercury species and RMC modeling of high-resolution diffraction data provide additional details on local Hg environment and connectivity implying the (HgS2/2), oligomeric chains (1 <= m <= 6) are acting as a network former while the HgS4/4-related mixed agglomerated units behave as a modifier. C1 [Kassem, M.; Sokolov, A.; Cuisset, A.; Khaoulani, S.; Masselin, P.; Bychkov, E.] Univ Littoral Cote dOpale, LPCA, EA CNRS 4493, F-59140 Dunkerque, France. [Usuki, T.] Yamagata Univ, Fac Sci, Yamagata 9908560, Japan. [Le Coq, D.] Univ Rennes 1, UMR CNRS 6226, Sci Chim Rennes, F-35042 Rennes, France. [Le Coq, D.] Univ Rennes 1, Verres & Ceram, F-35042 Rennes, France. [Neuefeind, J. C.; Feygenson, M.] Oak Ridge Natl Lab, Neutron Scattering Sci Directorate, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. [Hannon, A. C.] Rutherford Appleton Lab, ISIS Facil, Didcot OX11 0QX, Oxon, England. [Benmore, C. J.] Argonne Natl Lab, Xray Sci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Bychkov, E (reprint author), Univ Littoral Cote dOpale, LPCA, EA CNRS 4493, F-59140 Dunkerque, France. EM bychkov@univ-littoral.fr OI Benmore, Chris/0000-0001-7007-7749 FU Agence Nationale de la Recherche (ANR, France) [ANR-15-ASTR-0016-01]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; Science and Technology Facilities Council [RB1510269]; Office of Basic Energy Sciences, U.S. Department of Energy [DE-AC02-06CH1135] FX This work was supported by Agence Nationale de la Recherche (ANR, France) under Grant No. ANR-15-ASTR-0016-01. Research conducted at ORNL's Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. Experiments at the ISIS Pulsed Neutron and Muon Source were supported by a beamtime allocation (RB1510269) from the Science and Technology Facilities Council. Work at the Advanced Photon Source, Argonne National Laboratory, was supported in part by the Office of Basic Energy Sciences, U.S. Department of Energy, under Contract No. DE-AC02-06CH1135. NR 64 TC 0 Z9 0 U1 0 U2 3 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD JUN 16 PY 2016 VL 120 IS 23 BP 5278 EP 5290 DI 10.1021/acs.jpcb.6b03382 PG 13 WC Chemistry, Physical SC Chemistry GA DP0QS UT WOS:000378194900017 PM 27214120 ER PT J AU Ray, P Dohm, S Husch, T Schutter, C Persson, KA Balducci, A Kirchner, B Korth, M AF Ray, Promit Dohm, Sebastian Husch, Tamara Schuetter, Christoph Persson, Kristin A. Balducci, Andrea Kirchner, Barbara Korth, Martin TI Insights into Bulk Electrolyte Effects on the Operative Voltage of Electrochemical Double-Layer Capacitors SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID SPACE GAUSSIAN PSEUDOPOTENTIALS; DENSITY-FUNCTIONAL THEORY; SEMIEMPIRICAL QM METHODS; MOLECULAR-DYNAMICS; FORCE-FIELDS; BASIS-SETS; ORGANIC LIQUIDS; SUPERCAPACITORS; SOLVENTS; IDENTIFICATION AB Electrochemical double-layer capacitors (EDLCs) are robust, high-power, and fast-charging energy storage devices. Rational design of novel electrolyte materials could further improve the performance of EDLCs. Computational methods offer immense scope in aiding the development of such materials. Trends in experimentally observed operative voltages nevertheless remain difficult to predict and understand. We discuss here the intriguing case of adiponitrile (ADN) versus 2-methyl-glutaronitrile (2MGN) based electrolytes, which result in very different operative voltages in EDLCs despite structural similarity. As a preliminary step, bulk electrolyte effects on electrochemical stability are investigated by ab initio molecular dynamics (AIMD) and static, cluster-based quantum chemistry calculations. C1 [Ray, Promit; Kirchner, Barbara] Univ Bonn, Mulliken Ctr Theoret Chem, Beringstr 4 6, D-53115 Bonn, Germany. [Dohm, Sebastian; Husch, Tamara; Korth, Martin] Univ Ulm, Inst Theoret Chem, Albert Einstein Allee 11, D-89069 Ulm, Germany. [Schuetter, Christoph; Balducci, Andrea] Karlsruhe Inst Technol, Helmholtz Inst Ulm, Helmholtzstr 11, D-89081 Ulm, Germany. [Persson, Kristin A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Electrochem Technol Grp, 1 Cyclotron Rd MS 33R0146, Berkeley, CA 94720 USA. RP Korth, M (reprint author), Univ Ulm, Inst Theoret Chem, Albert Einstein Allee 11, D-89069 Ulm, Germany. EM martin.korth@uni-ulm.de FU Deutsche Forschungsgemeinschaft [KI786/8-1, SPP 1708, KI768/12-1]; Bundesministerium fur Bildung and Forschung (BMBF) within the project IES [03EK3010]; Barbara Mez-Starck Foundation; DFG [FOR1376]; Joint Center of Energy Storage Research (JCESR) an Energy Innovation Hub - U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-05CH11231]; bwHPC; bwHPC-C5 project through compute services of the JUSTUS HPC facility at the University of Ulm; Ministry of Science, Research and the Arts Baden-Wurttemberg; Germany Research Foundation (DFG) FX BK and PR would like to thank the support from the Deutsche Forschungsgemeinschaft under the KI786/8-1 project and the SPP 1708 project KI768/12-1. AB and CS would like to thank the Bundesministerium fur Bildung and Forschung (BMBF) within the project IES (contract number 03EK3010) for the financial support. MK, SD, and TH gratefully acknowledge financial support from the Barbara Mez-Starck Foundation and the DFG Research Unit FOR1376. KAP was funded by the Joint Center of Energy Storage Research (JCESR) an Energy Innovation Hub funded by the U.S. Department of Energy, Office of Basic Energy Sciences, under contract No. DE-AC02-05CH11231. This research was supported in part by the bwHPC initiative and the bwHPC-C5 project through compute services of the JUSTUS HPC facility at the University of Ulm. bwHPC and bwHPC-C5 (http://www.bwhpc-c5.de) are funded by the Ministry of Science, Research and the Arts Baden-Wurttemberg (MWK), and the Germany Research Foundation (DFG). NR 51 TC 3 Z9 3 U1 8 U2 20 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUN 16 PY 2016 VL 120 IS 23 BP 12325 EP 12336 DI 10.1021/acs.jpcc.6b00891 PG 12 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DP0RF UT WOS:000378196200001 ER PT J AU Garcia-Lastra, JM Boukahil, I Qiao, RM Rubio, A Himpsel, FJ AF Garcia-Lastra, J. M. Boukahil, Idris Qiao, Ruimin Rubio, Angel Himpsel, F. J. TI Electronic Structure of Low-Dimensional Carbon pi-Systems SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID EXCITON BINDING-ENERGIES; SENSITIZED SOLAR-CELLS; QUANTUM-WELL STATES; CONFIGURATION-INTERACTION; CHARGE SEPARATION; DENSITY; EXCITATIONS; MOLECULES; SPECTRA; APPROXIMATION AB X-ray absorption spectroscopy (XAS) is combined with density functional theory (DFT) to determine the orbitals of one- and two-dimensional carbon pi-systems (lycopene, beta-carotene, retinal, retinol, retinoic acid, coronene, triphenylene). Considerable fine structure is observed for the transition from the C is level to the lowest unoccupied molecular orbital (LUMO) and explained by DFT. The wave functions of the one-dimensional chain molecules display the node structure of a vibrating string. The XAS transition energy is decomposed into contributions from the C is core level, the pi* final state, and the electron hole interaction. For the latter, we develop a simple model that accurately represents a full Delta-self-consistent field (Delta SCF) calculation. The distortion of the LUMO because of its interaction with the C is hole is investigated. These results illustrate the electronic states of prototypical pi-bonded carbon structures with low-dimensional character, such as those used in molecular complexes for solar cells, confined graphene structures, and molecular wires. C1 [Garcia-Lastra, J. M.] Tech Univ Denmark, Dept Energy Convers & Storage, Fysjikvej 309, DK-2800 Lyngby, Denmark. [Boukahil, Idris; Himpsel, F. J.] Univ Wisconsin, Dept Phys, 1150 Univ Ave, Madison, WI 53706 USA. [Qiao, Ruimin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Rubio, Angel] Max Planck Inst Struct & Dynam Matter, Hamburg, Germany. [Rubio, Angel] Univ Basque Country, CFM CSIC UPV EHU MPC, NanoBio Spect Grp, San Sebastian 20018, Spain. [Rubio, Angel] Univ Basque Country, CFM CSIC UPV EHU MPC, ETSF, San Sebastian 20018, Spain. [Rubio, Angel] DIPC, San Sebastian 20018, Spain. RP Himpsel, FJ (reprint author), Univ Wisconsin, Dept Phys, 1150 Univ Ave, Madison, WI 53706 USA. EM fhimpsel@wisc.edu RI DONOSTIA INTERNATIONAL PHYSICS CTR., DIPC/C-3171-2014; Qiao, Ruimin/E-9023-2013; Rubio, Angel/A-5507-2008; Garcia Lastra, Juan Maria/A-9996-2010; CSIC-UPV/EHU, CFM/F-4867-2012 OI Rubio, Angel/0000-0003-2060-3151; Garcia Lastra, Juan Maria/0000-0001-5311-3656; FU NSF through the University of Wisconsin Materials Research Science and Engineering Center [DMR-1121288]; DOE (BES) [DE-AC02-05CH11231, DE-SC0006931]; Spanish Ministry of Economy and Competitiveness [FIS2012-30996, FIS2013-46159-C3-1-P]; Grupos Consolidados [IT578-13]; COST Action [MP1306] FX The help of Wanli Yang with the experiment is gratefully acknowledged. This research was supported by the NSF through the University of Wisconsin Materials Research Science and Engineering Center (DMR-1121288). We also acknowledge support by the DOE (BES) for the synchrotron radiation experiments at the Advanced Light Source (ALS) under the Contracts DE-AC02-05CH11231 (ALS) and DE-SC0006931 (endstation). J.M.G.L. acknowledges support from the Spanish Ministry of Economy and Competitiveness under Projects FIS2012-30996 and FIS2013-46159-C3-1-P, Grupos Consolidados (IT578-13), and COST Action MP1306 (EUSpec). NR 45 TC 0 Z9 0 U1 7 U2 15 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUN 16 PY 2016 VL 120 IS 23 BP 12362 EP 12368 DI 10.1021/acs.jpcc.6b02530 PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DP0RF UT WOS:000378196200005 ER PT J AU Schwenzer, B Kaspar, TC Shin, Y Gotthold, DW AF Schwenzer, Birgit Kaspar, Tiffany C. Shin, Yongsoon Gotthold, David W. TI Spectroscopic Study of Graphene Oxide Membranes Exposed to Ultraviolet Light SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID SURFACE FUNCTIONAL-GROUPS; X-RAY PHOTOELECTRON; GRAPHITE OXIDE; REDUCTION; WATER; NANOCOMPOSITES; NANOSHEETS; STATE AB Hierarchically stacked graphene oxide (GO) membranes have been observed to undergo physical and chemical changes under ambient conditions. In this study, the slow degradation of GO membranes is mimicked and accelerated by UV light (254 nm) exposure. Spectroscopic and X-ray diffraction analyses confirm that the observed changes, including macroscopic as well as atomic-scale, alterations, cannot be attributed to loss of intercalated water-molecules between the GO sheets, but UV light exposure triggers a partial reduction of the GO membrane to a more graphene-like material. C1 [Schwenzer, Birgit; Kaspar, Tiffany C.; Shin, Yongsoon] Pacific NW Natl Lab, Phys & Computat Sci Directorate, Richland, WA 99352 USA. [Gotthold, David W.] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. RP Gotthold, DW (reprint author), Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. EM David.Gotthold@pnnl.gov NR 38 TC 0 Z9 0 U1 9 U2 13 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUN 16 PY 2016 VL 120 IS 23 BP 12559 EP 12567 DI 10.1021/acs.jpcc.6b03033 PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DP0RF UT WOS:000378196200026 ER PT J AU Ho, JM Psciuk, BT Chase, HM Rudshteyn, B Upshur, MA Fu, L Thomson, RJ Wang, HF Geiger, FM Batista, VS AF Ho, Junming Psciuk, Brian T. Chase, Hilary M. Rudshteyn, Benjamin Upshur, Mary Alice Fu, Li Thomson, Regan J. Wang, Hong-Fei Geiger, Franz M. Batista, Victor S. TI Sum Frequency Generation Spectroscopy and Molecular Dynamics Simulations Reveal a Rotationally Fluid Adsorption State of alpha-Pinene on Silica SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID DENSITY-FUNCTIONAL THEORY; VIBRATIONAL SPECTROSCOPY; FORCE-FIELD; THEORETICAL-ANALYSIS; WATER-SURFACE; SFG-VS; DISPERSION CORRECTIONS; UNIFIED TREATMENT; LIQUID INTERFACE; ROOM-TEMPERATURE AB A rotationally fluid state of a-pinene at fused silica/vapor interfaces is revealed by computational and experimental vibrational sum frequency generation (SFG) studies. We report the first assignment of the vibrational modes in the notoriously congested C-H stretching region of a-pinene and identify its bridge methylene group on the four-membered ring ("(CH2)-C-beta") as the origin of its dominant spectral feature. We find that the spectra are perfused with Fermi resonances that need to be accounted for explicitly in the computation of vibrational spectra of strained hydrocarbons such as alpha-pinene. The preferred orientations of alpha-pinene are consistent with optimization of van der Waals contacts with the silica surface that results in a bimodal distribution of highly fluxional orientations in which the (CH2)-C-beta group points "towards" or "away from" the surface. Classical molecular dynamics simulations further provide rotational diffusion constants of 49 +/- 1 ps and 2580 +/- 60 ps, which are attributed to two broad types of adsorption modes on silica. The reported findings are particularly relevant to the exposure of alpha-pinene to primary oxidants in heterogeneous catalytic pathways that exploit alpha-pinene as a sustainable feedstock for fine chemicals and polymers. C1 [Ho, Junming; Psciuk, Brian T.; Rudshteyn, Benjamin; Batista, Victor S.] Yale Univ, Dept Chem, POB 208107, New Haven, CT 06520 USA. [Fu, Li; Wang, Hong-Fei] Pacific NW Natl Lab, William R Wiley Environm Mol Sci Lab, Richland, WA 99352 USA. [Chase, Hilary M.; Upshur, Mary Alice; Thomson, Regan J.; Geiger, Franz M.] Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. [Wang, Hong-Fei] Pacific NW Natl Lab, Div Phys Sci, POB 999, Richland, WA 99352 USA. [Ho, Junming] Inst High Performance Comp, 1 Fusionopolis Way,16-16 Connexis North, Singapore 138632, Singapore. RP Batista, VS (reprint author), Yale Univ, Dept Chem, POB 208107, New Haven, CT 06520 USA.; Geiger, FM (reprint author), Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. EM geigerf@chem.northwestern.edu; victor.batista@yale.edu RI Wang, Hongfei/B-1263-2010; Ho, Junming /A-1070-2012 OI Wang, Hongfei/0000-0001-8238-1641; Ho, Junming /0000-0001-9381-924X FU Agency for Science, Technology and Research (Singapore); National Science Foundation (NSF) Graduate Research Fellowship [DGE-1324585, DGE-1122492]; Institute for Sustainability and Energy at Northwestern (ISEN); National Aeronautics and Space Administration Earth and Space (NASA ESS) Fellowship; NSF [CHE-1212692, SP0017343, CHE-1465108]; U.S. Department of Energy's (DOE) Office of Biological and Environmental Research (BER) FX J.H. gratefully acknowledges support from the Agency for Science, Technology and Research (Singapore). H.M.C. gratefully acknowledges support from a National Science Foundation (NSF) Graduate Research Fellowship under Grant No. DGE-1324585 and the Institute for Sustainability and Energy at Northwestern (ISEN). B.R. gratefully acknowledges support from the NSF Graduate Research Fellowship under Grant No. DGE-1122492. M.A.U. gratefully acknowledges support from a National Aeronautics and Space Administration Earth and Space (NASA ESS) Fellowship and an NSF Graduate Research Fellowship. F.M.G. and R.J.T. acknowledge support from NSF Grants CHE-1212692 and SP0017343. V.S.B. acknowledges supercomputer time from NERSC and the Yale High Performance Computing Center and support from NSF Grant CHE-1465108. Part of this work was conducted at the William R. Wiley Environmental Molecular Sciences Laboratory (EMSL) under user ID 47891. EMSL is a national scientific user facility located at the Pacific Northwest National Laboratory and sponsored by the U.S. Department of Energy's (DOE) Office of Biological and Environmental Research (BER). NR 92 TC 2 Z9 2 U1 10 U2 23 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUN 16 PY 2016 VL 120 IS 23 BP 12578 EP 12589 DI 10.1021/acs.jpcc.6b03158 PG 12 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DP0RF UT WOS:000378196200028 ER PT J AU Mercado, R Vlaisayljevich, B Lin, LC Lee, K Lee, Y Mason, JA Xiao, DJ Gonzalez, MI Kapelewski, MT Neaton, JB Smit, B AF Mercado, Rocio Vlaisayljevich, Bess Lin, Li-Chiang Lee, Kyuho Lee, Yongjin Mason, Jarad A. Xiao, Dianne J. Gonzalez, Miguel I. Kapelewski, Matthew T. Neaton, Jeffrey B. Smit, Berend TI Force Field Development from Periodic Density Functional Theory Calculations for Gas Separation Applications Using Metal-Organic Frameworks SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID CARBON-DIOXIDE CAPTURE; ELECTRONIC-STRUCTURE CALCULATIONS; MOLECULAR-DYNAMICS SIMULATIONS; AUGMENTED-WAVE METHOD; CO2 ADSORPTION; POTENTIAL FUNCTIONS; WATER-ADSORPTION; LIQUID WATER; M-2(DOBDC) M; SITES AB We present accurate force fields developed from density functional theory (DFT) calculations with periodic boundary conditions for use in molecular simulations involving M-2(dobdc) (M-MOF-74; dobdc(4-) = 2,5-dioxidobenzenedicarboxylate; M = Mg, Mn, Fe, Co, Ni, Zn) and frameworks of similar topology. In these systems, conventional force fields fail to accurately model gas adsorption due to the strongly binding open-metal sites. The DFT-derived force fields predict the adsorption of CO2, H2O, and CH4 inside these frameworks much more accurately than other common force fields. We show that these force fields can also be used for M2(dobpdc) (dobpdc(4-) = 4,4'-dioxidobiphenyl-3,3'-dicarboxylate), an extended version of MOF-74, and thus are a promising alternative to common force fields for studying materials similar to MOF-74 for carbon capture applications. Furthermore, it is anticipated that the approach can be applied to other metal organic framework topologies to obtain force fields for different systems. We have used this force field to study the effect of contaminants such as H2O and N-2 upon these materials' performance for the separation of CO2 from the emissions of natural gas reservoirs and coal-fired power plants. Specifically, mixture adsorption isotherms calculated with these DFT-derived force fields showed a significant reduction in the uptake of many gas components in the presence of even trace amounts of H2O vapor. The extent to which the various gases are affected by the concentration of H2O in the reservoir is quantitatively different for the different frameworks and is related to their heats of adsorption. Additionally, significant increases in CO2 selectivities over CH4 and N2 are observed as the temperature of the systems is lowered. C1 [Mercado, Rocio; Mason, Jarad A.; Xiao, Dianne J.; Gonzalez, Miguel I.; Kapelewski, Matthew T.; Smit, Berend] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Vlaisayljevich, Bess; Lin, Li-Chiang; Lee, Kyuho; Smit, Berend] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Neaton, Jeffrey B.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Lee, Kyuho; Neaton, Jeffrey B.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Lee, Kyuho] Synopsys Inc, Mountain View, CA 94043 USA. [Lee, Yongjin; Smit, Berend] Ecole Polytech Fed Lausanne, Valais, Inst Sci & Ingn Chim, Rue Ind 17, CH-1951 Sion, Switzerland. RP Smit, B (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Smit, B (reprint author), Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA.; Smit, B (reprint author), Ecole Polytech Fed Lausanne, Valais, Inst Sci & Ingn Chim, Rue Ind 17, CH-1951 Sion, Switzerland. EM berend-smit@berkeley.edu RI Smit, Berend/B-7580-2009; Lin, Li-Chiang/J-8120-2014; OI Smit, Berend/0000-0003-4653-8562; Gonzalez, Miguel/0000-0003-4250-9035 FU Center for Gas Separations Relevant to Clean Energy Technologies; Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001015]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; NSF Graduate Research Fellowships FX This material is based upon work supported as part of the Center for Gas Separations Relevant to Clean Energy Technologies, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under award number DE-SC0001015. Work at the Molecular Foundry was supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under contract no. DE-AC02-05CH11231. This research used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Work at the Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under contract no. DE-AC02-05CH11231. R.M. and M.T.K. acknowledge support from NSF Graduate Research Fellowships. In addition, we thank Jeffrey R. Long for helpful comments and discussions. NR 66 TC 4 Z9 4 U1 25 U2 56 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUN 16 PY 2016 VL 120 IS 23 BP 12590 EP 12604 DI 10.1021/acs.jpcc.6b03393 PG 15 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DP0RF UT WOS:000378196200029 ER PT J AU Yu, XJ Zhang, ZR Yang, CW Bebensee, F Heissler, S Nefedov, A Tang, MR Ge, QF Chen, L Kay, BD Dohnalek, Z Wang, YM Woll, C AF Yu, Xiaojuan Zhang, Zhenrong Yang, Chengwu Bebensee, Fabian Heissler, Stefan Nefedov, Alexei Tang, Miru Ge, Qingfeng Chen, Long Kay, Bruce D. Dohnalek, Zdenek Wang, Yuemin Woell, Christof TI Interaction of Formaldehyde with the Rutile TiO2(110) Surface: A Combined Experimental and Theoretical Study SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID INITIO MOLECULAR-DYNAMICS; TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; METHANOL OXIDATION; TITANIUM-DIOXIDE; OXIDE SURFACES; ACTIVE-SITES; SOLID FORMALDEHYDE; LOSS SPECTROSCOPY; O-2 DISSOCIATION AB The adsorption and reaction of formaldehyde (CH2O) on the oxidized rutile TiO2(110) surface were studied by temperature-programmed desorption (TPD), scanning tunneling microscopy (STM), infrared reflection absorption spectroscopy (IRRAS), and density functional theory (DFT) calculations. The experimental and theoretical data reveal the presence of various species depending on the temperature and coverage. Exposure to formaldehyde at 65 K leads to the formation of CH2O multilayers, which desorb completely upon heating to 120 K. After smaller exposures at low temperatures (45-65 K), STM allowed us to identify individual, isolated CH2O monomers. The, theoretical results indicate that these monomers are bound to the surface Ti-5c sites via sigma-donation and adopt a tilted geometry. Upon heating, the CH2O monomers polymerize to form paraformaldehyde (polyoxymethylene, POM) chains, oriented primarily along the Ti-5c rows ([001] direction). Upon further heating, POM is found to decompose around 250 K, releasing CH2O into the gas phase. In addition, dioxymethylene (DOM) was detected as minority species formed via reaction of Ti-5c-bound CH2O with surface O atoms. For all substrate species, the characteristic IR vibrations were measured. Because these are the first IRRAS data for TiO2 macroscopic single crystals exposed to formaldehyde, we have performed DFT calculations to aid the assignment of the various bands. C1 [Yu, Xiaojuan; Yang, Chengwu; Bebensee, Fabian; Heissler, Stefan; Nefedov, Alexei; Wang, Yuemin; Woell, Christof] Karlsruhe Inst Technol, Inst Funct Interfaces, D-76344 Eggenstein Leopoldshafen, Germany. [Zhang, Zhenrong] Baylor Univ, Dept Phys, Waco, TX 76798 USA. [Tang, Miru; Ge, Qingfeng] So Illinois Univ, Dept Chem & Biochem, Carbondale, IL 62901 USA. [Chen, Long; Kay, Bruce D.; Dohnalek, Zdenek] Pacific NW Natl Lab, Phys & Computat Sci Directorate, Richland, WA 99354 USA. [Chen, Long; Kay, Bruce D.; Dohnalek, Zdenek] Pacific NW Natl Lab, Inst Interfacial Catalysis, Richland, WA 99354 USA. RP Wang, YM; Woll, C (reprint author), Karlsruhe Inst Technol, Inst Funct Interfaces, D-76344 Eggenstein Leopoldshafen, Germany. EM yuemin.wang@kit.edu; christofwoell@kit.edu RI Ge, Qingfeng/A-8498-2009; Woll, Christof/D-5563-2011 OI Ge, Qingfeng/0000-0001-6026-6693; Woll, Christof/0000-0003-1078-3304 FU "Science and Technology of Nano systems" Programme [432202]; China Scholarship Council (CSC); Helmholtz Research School "Energy-related catalysis"; NSF-CBET program [CBET-1438440]; US Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences Biosciences [KC0301050-47319]; Department of Energy's Office of Biological and Environmental Research at Pacific Northwest National Laboratory (PNNL) FX The funding from the "Science and Technology of Nano systems" Programme (project no. 432202) is gratefully acknowledged. X.Y. and C.Y. are grateful for Ph.D. fellowships donated by the China Scholarship Council (CSC). C.Y. thanks the Helmholtz Research School "Energy-related catalysis" for financial support. M.T. and Q.G. acknowledge the support of NSF-CBET program (award no. CBET-1438440). L.C., Z.D., and B.D.K. acknowledge support by the US Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences & Biosciences, under grant KC0301050-47319. The TPD and STM experiments were performed in EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory (PNNL). PNNL is a multiprogram national laboratory operated for DOE by Battelle. NR 71 TC 2 Z9 2 U1 24 U2 65 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUN 16 PY 2016 VL 120 IS 23 BP 12626 EP 12636 DI 10.1021/acs.jpcc.6b03689 PG 11 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DP0RF UT WOS:000378196200033 ER PT J AU Liddick, SN Spyrou, A Crider, BP Naqvi, F Larsen, AC Guttormsen, M Mumpower, M Surman, R Perdikakis, G Bleuel, DL Couture, A Campo, LC Dombos, AC Lewis, R Mosby, S Nikas, S Prokop, CJ Renstrom, T Rubio, B Siem, S Quinn, SJ AF Liddick, S. N. Spyrou, A. Crider, B. P. Naqvi, F. Larsen, A. C. Guttormsen, M. Mumpower, M. Surman, R. Perdikakis, G. Bleuel, D. L. Couture, A. Campo, L. Crespo Dombos, A. C. Lewis, R. Mosby, S. Nikas, S. Prokop, C. J. Renstrom, T. Rubio, B. Siem, S. Quinn, S. J. TI Experimental Neutron Capture Rate Constraint Far from Stability SO PHYSICAL REVIEW LETTERS LA English DT Article ID R-PROCESS NUCLEOSYNTHESIS; LEVEL DENSITY; STAR MERGERS; STRENGTH FUNCTION; NUCLEAR-PHYSICS; IMPACT; MODEL; ASTROPHYSICS; SYSTEMATICS; SPECTRA AB Nuclear reactions where an exotic nucleus captures a neutron are critical for a wide variety of applications, from energy production and national security, to astrophysical processes, and nucleosynthesis. Neutron capture rates are well constrained near stable isotopes where experimental data are available; however, moving far from the valley of stability, uncertainties grow by orders of magnitude. This is due to the complete lack of experimental constraints, as the direct measurement of a neutron-capture reaction on a short-lived nucleus is extremely challenging. Here, we report on the first experimental extraction of a neutron capture reaction rate on Ni-69, a nucleus that is five neutrons away from the last stable isotope of Ni. The implications of this measurement on nucleosynthesis around mass 70 are discussed, and the impact of similar future measurements on the understanding of the origin of the heavy elements in the cosmos is presented. C1 [Liddick, S. N.; Spyrou, A.; Crider, B. P.; Naqvi, F.; Perdikakis, G.; Dombos, A. C.; Lewis, R.; Prokop, C. J.; Quinn, S. J.] Michigan State Univ, Natl Supercond Cyclotron Lab, E Lansing, MI 48824 USA. [Liddick, S. N.; Lewis, R.; Prokop, C. J.] Michigan State Univ, Dept Chem, E Lansing, MI 48824 USA. [Spyrou, A.; Dombos, A. C.; Quinn, S. J.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Spyrou, A.; Perdikakis, G.; Dombos, A. C.; Nikas, S.; Quinn, S. J.] Michigan State Univ, Joint Inst Nucl Astrophys, E Lansing, MI 48824 USA. [Larsen, A. C.; Guttormsen, M.; Campo, L. Crespo; Renstrom, T.; Siem, S.] Univ Oslo, Dept Phys, N-0316 Oslo, Norway. [Mumpower, M.; Surman, R.] Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. [Mumpower, M.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87544 USA. [Perdikakis, G.; Nikas, S.] Cent Michigan Univ, Mt Pleasant, MI 48859 USA. [Bleuel, D. L.] Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. [Couture, A.; Mosby, S.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. [Rubio, B.] Univ Valencia, CSIC, IFIC, Valencia 46071, Spain. RP Liddick, SN (reprint author), Michigan State Univ, Natl Supercond Cyclotron Lab, E Lansing, MI 48824 USA.; Liddick, SN (reprint author), Michigan State Univ, Dept Chem, E Lansing, MI 48824 USA. RI Perdikakis, Georgios/K-4525-2014; Larsen, Ann-Cecilie/C-8742-2014 OI Perdikakis, Georgios/0000-0002-8539-8737; Larsen, Ann-Cecilie/0000-0002-2188-3709 FU Michigan State University; NSF [PHY-1102511, 1350234, 1430152, 0822648, 1419765]; U.S. Department of Energy [DE-SC0013039, DE-AC52-07NA27344]; National Nuclear Security Administration [DE-NA0000979, DE-FC03-03NA00143]; College of Science and Technology of Central Michigan University; Facility for Rare Isotope Beams FX This research was supported by Michigan State University and the Facility for Rare Isotope Beams and was funded in part by the NSF under Contracts No. PHY-1102511 (NSCL), No. 1350234 (CAREER), No. 1430152 (JINA-CEE), No. 0822648, and No. 1419765 (M. M. and R. S.), and the U.S. Department of Energy under Contracts No. DE-SC0013039 (R. S.), No. DE-AC52-07NA27344 (LLNL), and the National Nuclear Security Administration under Award No. DE-NA0000979 and Grant No. DE-FC03-03NA00143. G. P. would like to acknowledge support from the College of Science and Technology of Central Michigan University. NR 50 TC 4 Z9 4 U1 6 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUN 16 PY 2016 VL 116 IS 24 AR 242502 DI 10.1103/PhysRevLett.116.242502 PG 6 WC Physics, Multidisciplinary SC Physics GA DO8UE UT WOS:000378058700003 PM 27367386 ER PT J AU Nunez, JK Bai, L Harrington, LB Hinder, TL Doudna, JA AF Nunez, James K. Bai, Lawrence Harrington, Lucas B. Hinder, Tracey L. Doudna, Jennifer A. TI CRISPR Immunological Memory Requires a Host Factor for Specificity SO MOLECULAR CELL LA English DT Article ID CAS ADAPTIVE IMMUNITY; NUCLEOID-ASSOCIATED PROTEINS; ESCHERICHIA-COLI; RETROVIRAL INTEGRATION; SPACER ACQUISITION; DNA-BINDING; MECHANISTIC BASIS; FOREIGN DNA; REPEATS; SITES AB Bacteria and archaea employ adaptive immunity against foreign genetic elements using CRISPR-Cas systems. To generate immunological memory, the Cas1-Cas2 protein complex captures 30-40 base pair segments of foreign DNA and catalyzes their integration into the host genome as unique spacer sequences. Although spacers are inserted strictly at the A-T-rich leader end of CRISPR loci in vivo, the molecular mechanism of leader-specific spacer integration remains poorly understood. Here we show that the E. coli integration host factor (IHF) protein is required for spacer acquisition in vivo and for integration into linear DNA in vitro. IHF binds to the leader sequence and induces a sharp DNA bend, allowing the Cas1Cas2 integrase to catalyze the first integration reaction at the leader-repeat border. Together, these results reveal that Cas1-Cas2-mediated spacer integration requires IHF-induced target DNA bending and explain the elusive role of CRISPR leader sequences during spacer acquisition. C1 [Nunez, James K.; Harrington, Lucas B.; Doudna, Jennifer A.] Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA. [Bai, Lawrence] Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. [Hinder, Tracey L.; Doudna, Jennifer A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Doudna, Jennifer A.] Univ Calif Berkeley, Innovat Genom Initiat, Berkeley, CA 94720 USA. [Doudna, Jennifer A.] Univ Calif Berkeley, Ctr RNA Syst Biol, Berkeley, CA 94720 USA. [Doudna, Jennifer A.] Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA. [Doudna, Jennifer A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Biophys & Integrated Bioimaging, Phys Biosci Div, Berkeley, CA 94720 USA. RP Doudna, JA (reprint author), Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA.; Doudna, JA (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Doudna, JA (reprint author), Univ Calif Berkeley, Innovat Genom Initiat, Berkeley, CA 94720 USA.; Doudna, JA (reprint author), Univ Calif Berkeley, Ctr RNA Syst Biol, Berkeley, CA 94720 USA.; Doudna, JA (reprint author), Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA.; Doudna, JA (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Biophys & Integrated Bioimaging, Phys Biosci Div, Berkeley, CA 94720 USA. EM doudna@berkeley.edu FU U.S. National Science Foundation [1244557]; NIH [S10RR029668, S10RR027303]; U.S. National Science Foundation; UC Berkeley Chancellor's Graduate Fellowship; UC Berkeley SURF Rose Hills Fellowship FX We thank A. Lee and D. Burstein for assisting with deep-sequencing data analysis and M. Davis for providing reagents to generate the knockout strains. We are grateful to A. Engelman (Harvard), A. Wright, and J.A.D. lab members for helpful discussions. This project was funded by U.S. National Science Foundation grant No. 1244557 to J.A.D. This work used the Vincent J. Coates Genomics Sequencing Laboratory at UC Berkeley, supported by NIH S10 Instrumentation Grants S10RR029668 and S10RR027303. J.K.N. and L.B.H. are supported by U.S. National Science Foundation Graduate Fellowships and J.K.N. by a UC Berkeley Chancellor's Graduate Fellowship. L.B. acknowledges support from a UC Berkeley SURF Rose Hills Fellowship. J.A.D. is an Investigator of the Howard Hughes Medical Institute. The authors have filed a related patent; J.A.D. is a co-founder and Scientific Advisory Board member of Caribou Biosciences and Intellia Therapeutics and a co-founder of Editas Medicine. NR 36 TC 7 Z9 7 U1 4 U2 14 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 1097-2765 EI 1097-4164 J9 MOL CELL JI Mol. Cell PD JUN 16 PY 2016 VL 62 IS 6 BP 824 EP 833 DI 10.1016/j.molcel.2016.04.027 PG 10 WC Biochemistry & Molecular Biology; Cell Biology SC Biochemistry & Molecular Biology; Cell Biology GA DP1BI UT WOS:000378224900005 PM 27211867 ER PT J AU Das, AK Vemuri, RS Kutnyakov, I McGrail, BP Motkuri, RK AF Das, Atanu Kumar Vemuri, Rama Sesha Kutnyakov, Igor McGrail, B. Peter Motkuri, Radha Kishan TI An Efficient Synthesis Strategy for Metal-Organic Frameworks: Dry-Gel Synthesis of MOF-74 Framework with High Yield and Improved Performance SO SCIENTIFIC REPORTS LA English DT Article ID ASSISTED CRYSTALLIZATION; COORDINATION POLYMER; GAS-ADSORPTION; SEPARATION; SITES; PORES; CHEMISTRY; ZEOLITE; XENON AB Vapor-assisted dry-gel synthesis of the metal-organic framework-74 (MOF-74) structure, specifically Ni-MOF-74 produced from synthetic precursors using an organic-water hybrid solvent system, showed a very high yield (>90% with respect to 2,5-dihydroxyterepthalic acid) and enhanced performance. The Ni-MOF-74 obtained showed improved sorption characteristics towards CO2 and the refrigerant fluorocarbon dichlorodifluoromethane. Unlike conventional synthesis, which takes 72 hours using the tetrahydrofuran-water system, this kinetic study showed that Ni-MOF-74 forms within 12 hours under dry-gel conditions with similar performance characteristics, and exhibits its best performance characteristics even after 24 hours of heating. In the dry-gel conversion method, the physical separation of the solvent and precursor mixture allows for recycling of the solvent. We demonstrated efficient solvent recycling (up to three times) that resulted in significant cost benefits. The scaled-up manufacturing cost of Ni-MOF-74 synthesized via our dry-gel method is 45% of conventional synthesis cost. Thus, for bulk production of the MOFs, the proposed vapor-assisted, dry-gel method is efficient, simple, and inexpensive when compared to the conventional synthesis method. C1 [Das, Atanu Kumar; Kutnyakov, Igor] Pacific NW Natl Lab, Div Phys Sci, Ctr Mol Electrocatalysis, Richland, WA 99352 USA. [Vemuri, Rama Sesha; McGrail, B. Peter; Motkuri, Radha Kishan] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. RP Motkuri, RK (reprint author), Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. EM radhakishan.motkuri@pnnl.gov RI Motkuri, Radha/F-1041-2014 OI Motkuri, Radha/0000-0002-2079-4798 FU Laboratory Directed Research and Development at Pacific Northwest National Laboratory (PNNL); U.S. Department of Energy (DOE), Energy Efficiency and Renewable Energy's Geothermal Technologies Office (GTO); U.S. Department of Energy (DOE) [DE-AC05-76RL01830] FX Acknowledgements This work was supported by Laboratory Directed Research and Development funding at Pacific Northwest National Laboratory (PNNL) and U.S. Department of Energy (DOE), Energy Efficiency and Renewable Energy's Geothermal Technologies Office (GTO). PNNL is operated by Battelle for the U.S. Department of Energy (DOE) under Contract DE-AC05-76RL01830. NR 42 TC 4 Z9 4 U1 48 U2 122 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JUN 16 PY 2016 VL 6 AR 28050 DI 10.1038/srep28050 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DO9BG UT WOS:000378078700001 PM 27306598 ER PT J AU Ho, TA Criscenti, LJ Wang, YF AF Tuan Anh Ho Criscenti, Louise J. Wang, Yifeng TI Nanostructural control of methane release in kerogen and its implications to wellbore production decline SO SCIENTIFIC REPORTS LA English DT Article ID NUCLEAR-MAGNETIC-RESONANCE; HIGH-PRESSURE ADSORPTION; MOLECULAR SIMULATION; ORGANIC-MATTER; GAS SHALE; CARBON-DIOXIDE; SURFACE-AREA; SYSTEMS; COAL; SEPARATION AB Despite massive success of shale gas production in the US in the last few decades there are still major concerns with the steep decline in wellbore production and the large uncertainty in a long-term projection of decline curves. A reliable projection must rely on a mechanistic understanding of methane release in shale matrix-a limiting step in shale gas extraction. Using molecular simulations, we here show that methane release in nanoporous kerogen matrix is characterized by fast release of pressurized free gas (accounting for similar to 30-47% recovery) followed by slow release of adsorbed gas as the gas pressure decreases. The first stage is driven by the gas pressure gradient while the second stage is controlled by gas desorption and diffusion. We further show that diffusion of all methane in nanoporous kerogen behaves differently from the bulk phase, with much smaller diffusion coefficients. The MD simulations also indicate that a significant fraction (3-35%) of methane deposited in kerogen can potentially become trapped in isolated nanopores and thus not recoverable. Our results shed a new light on mechanistic understanding gas release and production decline in unconventional reservoirs. The long-term production decline appears controlled by the second stage of gas release. C1 [Tuan Anh Ho; Criscenti, Louise J.] Sandia Natl Labs, Dept Geochem, POB 5800, Albuquerque, NM 87185 USA. [Wang, Yifeng] Sandia Natl Labs, Nucl Waste Disposal Res & Anal Dept, POB 5800, Albuquerque, NM 87185 USA. RP Criscenti, LJ (reprint author), Sandia Natl Labs, Dept Geochem, POB 5800, Albuquerque, NM 87185 USA. EM ljcrisc@sandia.gov FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; Sandia National Laboratories LDRD (Laboratory Directed Research and Development) project through Geoscience Research Foundation; National Energy Technology Laboratory project FX Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. This research was funded by a Sandia National Laboratories LDRD (Laboratory Directed Research and Development) project through Geoscience Research Foundation and by a National Energy Technology Laboratory project (both to Y. Wang). Discussions and initial literature searches with organic geochemist Dr. Mark Rigali provided the starting point for this research. The authors would like to thank Dr. Jeffrey Greathouse at Sandia National Laboratories for discussions regarding GCMC methodology and Dr. Susan Altman at Sandia National Laboratories for her constructive comments on an early draft of the manuscript. NR 52 TC 3 Z9 3 U1 15 U2 25 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JUN 16 PY 2016 VL 6 AR 28053 DI 10.1038/srep28053 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DO9BG UT WOS:000378078700004 PM 27306967 ER PT J AU Tashkandy, N Sabban, S Fakieh, M Meier-Kolthoff, JP Huang, SX Tindall, BJ Rohde, M Baeshen, MN Baeshen, NA Lapidus, A Copeland, A Pillay, M Reddy, TBK Huntemann, M Pati, A Ivanova, N Markowitz, V Woyke, T Goker, M Klenk, HP Kyrpides, NC Hahnke, RL AF Tashkandy, Nisreen Sabban, Sari Fakieh, Mohammad Meier-Kolthoff, Jan P. Huang, Sixing Tindall, Brian J. Rohde, Manfred Baeshen, Mohammed N. Baeshen, Nabih A. Lapidus, Alla Copeland, Alex Pillay, Manoj Reddy, T. B. K. Huntemann, Marcel Pati, Amrita Ivanova, Natalia Markowitz, Victor Woyke, Tanja Goeker, Markus Klenk, Hans-Peter Kyrpides, Nikos C. Hahnke, Richard L. TI High-quality draft genome sequence of Flavobacterium suncheonense GH29-5(T) (DSM 17707(T)) isolated from greenhouse soil in South Korea, and emended description of Flavobacterium suncheonense GH29-5(T) SO STANDARDS IN GENOMIC SCIENCES LA English DT Article DE Aerobic; Gliding motility; Greenhouse soil; Flavobacteriaceae; Bacteroidetes; GEBA; KMG-1; Tree of Life; GGDC; Carbohydrate active enzyme; Polysaccharide utilization loci ID STANDARD OPERATING PROCEDURE; SIMILARITY SEARCH TOOL; SP-NOV.; MARINE PROTEOBACTERIA; GENUS FLAVOBACTERIUM; ANNOTATION; DATABASE; ENZYMES; BACTEROIDES; PROPOSAL AB Flavobacterium suncheonense is a member of the family Flavobacteriaceae in the phylum Bacteroidetes. Strain GH29-5(T) (DSM 17707(T)) was isolated from greenhouse soil in Suncheon, South Korea. F. suncheonense GH29-5(T) is part of the Genomic Encyclopedia of Bacteria and Archaea project. The 2,880,663 bp long draft genome consists of 54 scaffolds with 2739 protein-coding genes and 82 RNA genes. The genome of strain GH29-5(T) has 117 genes encoding peptidases but a small number of genes encoding carbohydrate active enzymes (51 CAZymes). Metallo and serine peptidases were found most frequently. Among CAZymes, eight glycoside hydrolase families, nine glycosyl transferase families, two carbohydrate binding module families and four carbohydrate esterase families were identified. Suprisingly, polysaccharides utilization loci (PULs) were not found in strain GH29-5(T). Based on the coherent physiological and genomic characteristics we suggest that F. suncheonense GH29-5(T) feeds rather on proteins than saccharides and lipids. C1 [Tashkandy, Nisreen; Sabban, Sari; Fakieh, Mohammad; Baeshen, Mohammed N.; Baeshen, Nabih A.; Kyrpides, Nikos C.] King Abdulaziz Univ, Fac Sci, Dept Biol Sci, Jeddah 21413, Saudi Arabia. [Meier-Kolthoff, Jan P.; Huang, Sixing; Tindall, Brian J.; Goeker, Markus; Hahnke, Richard L.] Leibniz Inst DSMZ German Collect Microorganisms &, Braunschweig, Germany. [Rohde, Manfred] HZI Helmholtz Ctr Infect Res, Braunschweig, Germany. [Baeshen, Mohammed N.; Baeshen, Nabih A.] King Abdulaziz Univ, Ctr Nanotechnol, Jeddah 21413, Saudi Arabia. [Lapidus, Alla] St Petersburg State Univ, Ctr Algorithm Biotechnol, St Petersburg 199034, Russia. [Copeland, Alex; Reddy, T. B. K.; Huntemann, Marcel; Pati, Amrita; Ivanova, Natalia; Woyke, Tanja; Kyrpides, Nikos C.] Joint Genome Inst, Genome Biol Program, Dept Energy, Walnut Creek, CA USA. [Pillay, Manoj; Markowitz, Victor] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Biol Data Management & Technol Ctr, Berkeley, CA 94720 USA. [Klenk, Hans-Peter] Newcastle Univ, Sch Biol, Newcastle Upon Tyne NE1 7RU, Tyne & Wear, England. RP Tashkandy, N (reprint author), King Abdulaziz Univ, Fac Sci, Dept Biol Sci, Jeddah 21413, Saudi Arabia. EM ntashkandy@yahoo.com RI Kyrpides, Nikos/A-6305-2014; Faculty of, Sciences, KAU/E-7305-2017; Fac Sci, KAU, Biol Sci Dept/L-4228-2013; Lapidus, Alla/I-4348-2013; OI Kyrpides, Nikos/0000-0002-6131-0462; Lapidus, Alla/0000-0003-0427-8731; Meier-Kolthoff, Jan Philipp/0000-0001-9105-9814; Ivanova, Natalia/0000-0002-5802-9485 FU US Department of Energy's Office of Science, Biological and Environmental Research Program; University of California, Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; St. Petersburg State University grant [1.38.253.2015]; Bundesministerium fur Ernahrung und Landwirtschaft [22016812]; Center of Nanotechnology at King Abdulaziz University FX The authors gratefully acknowledge the help of Andrea Schutze for growing cells of GH29-5T and of Evelyne-Marie Brambilla (both at DSMZ), for DNA extraction and quality control. This work was performed under the auspices of the US Department of Energy's Office of Science, Biological and Environmental Research Program, and by the University of California, Lawrence Berkeley National Laboratory under contract No. DE-AC02-05CH11231. AL was supported by the St. Petersburg State University grant (No 1.38.253.2015). R.L.H. was supported by the Bundesministerium fur Ernahrung und Landwirtschaft No. 22016812 (PI Brian J. Tindall). We would also like to thank the Center of Nanotechnology at King Abdulaziz University for their support. NR 65 TC 1 Z9 1 U1 1 U2 7 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1944-3277 J9 STAND GENOMIC SCI JI Stand. Genomic Sci. PD JUN 16 PY 2016 VL 11 AR 42 DI 10.1186/s40793-016-0159-5 PG 10 WC Genetics & Heredity; Microbiology SC Genetics & Heredity; Microbiology GA DO7HM UT WOS:000377953200001 PM 27313837 ER PT J AU Poutsma, ML Scientist, G AF Poutsma, Marvin L. Scientist, Guest TI Comment on "Radicalicity: A scale to compare reactivities of radicals" (Chem. Phys. Lett. 618 (2015) 99-101) SO CHEMICAL PHYSICS LETTERS LA English DT Editorial Material ID HYDROGEN ABSTRACTION REACTION; CHLORINE ATOM; EVOLUTION AB The recently proposed term "radicalicity" was described as a measure of the reactivity of a free radical Q(center dot), i.e., a kinetic quantity. It is shown here that in fact it is simply a frame-shifted version of the well-known bond dissociation energy, a thermodynamic quantity. Hence its use is discouraged. (C) 2016 Elsevier B.V. All rights reserved. C1 [Poutsma, Marvin L.; Scientist, Guest] Oak Ridge Natl Lab, Div Chem Sci, POB 2008, Oak Ridge, TN 37831 USA. RP Poutsma, ML (reprint author), Oak Ridge Natl Lab, Div Chem Sci, POB 2008, Oak Ridge, TN 37831 USA. EM poutsmaml@ornl.gov NR 10 TC 0 Z9 0 U1 1 U2 122 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2614 EI 1873-4448 J9 CHEM PHYS LETT JI Chem. Phys. Lett. PD JUN 16 PY 2016 VL 654 BP 139 EP 140 DI 10.1016/j.cplett.2016.04.034 PG 2 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DN6TS UT WOS:000377209800026 ER PT J AU Hou, BY Kim, S Kim, T Kim, J Hong, S Bahn, CB Park, C Kim, JH AF Hou, Binyang Kim, Seunghyun Kim, Taeho Kim, Jongjin Hong, Seungbum Bahn, Chi Bum Park, Changyong Kim, Ji Hyun TI The Hydration Structure at Yttria-Stabilized Cubic Zirconia (110)-Water Interface with Sub-Angstrom Resolution SO SCIENTIFIC REPORTS LA English DT Article ID X-RAY REFLECTIVITY; NEUTRON-SCATTERING; HYDROTHERMAL DEGRADATION; SURFACE-WATER; ZRO2; ADSORPTION; DYNAMICS; OXIDE; NANOPARTICLES; ELECTROLYTE AB The interfacial hydration structure of yttria-stabilized cubic zirconia (110) surface in contact with water was determined with similar to 0.5 angstrom resolution by high-resolution X-ray reflectivity measurement. The terminal layer shows a reduced electron density compared to the following substrate lattice layers, which indicates there are additional defects generated by metal depletion as well as intrinsic oxygen vacancies, both of which are apparently filled by water species. Above this top surface layer, two additional adsorbed layers are observed forming a characteristic interfacial hydration structure. The first adsorbed layer shows abnormally high density as pure water and likely includes metal species, whereas the second layer consists of pure water. The observed interfacial hydration structure seems responsible for local equilibration of the defective surface in water and eventually regulating the long-term degradation processes. The multitude of water interactions with the zirconia surface results in the complex but highly ordered interfacial structure constituting the reaction front. C1 [Hou, Binyang; Park, Changyong] Carnegie Inst Sci, Geophys Lab, High Pressure Collaborat Access Team, Argonne, IL 60439 USA. [Kim, Seunghyun; Kim, Taeho; Kim, Ji Hyun] Ulsan Natl Inst Sci & Technol, Sch Mech & Nucl Engn, Dept Nucl Sci & Engn, Ulsan 44919, South Korea. [Kim, Jongjin; Hong, Seungbum] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Hong, Seungbum] Korea Adv Inst Sci & Technol, Dept Mat Sci & Engn, Daejeon 34141, South Korea. [Bahn, Chi Bum] Pusan Natl Univ, Sch Mech Engn, Pusan 46241, South Korea. RP Park, C (reprint author), Carnegie Inst Sci, Geophys Lab, High Pressure Collaborat Access Team, Argonne, IL 60439 USA.; Kim, JH (reprint author), Ulsan Natl Inst Sci & Technol, Sch Mech & Nucl Engn, Dept Nucl Sci & Engn, Ulsan 44919, South Korea. EM cpark@carnegiescience.edu; kimjh@unist.ac.kr RI Hong, Seungbum/B-7708-2009; Park, Changyong/A-8544-2008; OI Hong, Seungbum/0000-0002-2667-1983; Park, Changyong/0000-0002-3363-5788; Hou, Binyang/0000-0003-0535-7706 FU International Collaborative Energy Technology R&D Program of the Korea Institute of Energy Technology Evaluation and Planning (KETEP) from the Ministry of Trade Industry and Energy [20138530030010]; High Pressure Collaborative Access Team (HPCAT) - DOE-NNSA [DE-NA0001974]; DOE-BES [DE-FG02-99ER45775]; DOE Office of Science by Argonne National Laboratory [DE-AC02-06CH11357] FX The work was performed under the auspices of the International Collaborative Energy Technology R&D Program (No. 20138530030010) of the Korea Institute of Energy Technology Evaluation and Planning (KETEP) granted financial resource from the Ministry of Trade Industry and Energy. CP and BH acknowledge support from High Pressure Collaborative Access Team (HPCAT), supported by DOE-NNSA under Award No. DE-NA0001974 and DOE-BES under Award No. DE-FG02-99ER45775. The Advanced Photon Source is a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. Authors thank Drs. Z. Zhang, E. Karapetrova and C.M. Schlepuetz at the APS Sector 33, C. Kenney-Benson at HPCAT, and Drs. S. Lee and Y. Kim at 9C of PLS for their technical supports. Authors also thank Drs. Guoyin Shen and Russell J. Hemley at Geophysical Laboratory of Carnegie Institution of Washington for their illuminative discussions and comments. Authors also thank the anonymous reviewers. NR 44 TC 1 Z9 1 U1 3 U2 3 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JUN 15 PY 2016 VL 6 AR 27916 DI 10.1038/srep27916 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DY3FI UT WOS:000384975800001 PM 27302473 ER PT J AU Rodriguez, JN Zhu, C Duoss, EB Wilson, TS Spadaccini, CM Lewicki, JP AF Rodriguez, Jennifer N. Zhu, Cheng Duoss, Eric B. Wilson, Thomas S. Spadaccini, Christopher M. Lewicki, James P. TI Shape-morphing composites with designed micro-architectures SO SCIENTIFIC REPORTS LA English DT Article ID EPOXIDIZED SOYBEAN OIL; MEMORY POLYMERS; RENEWABLE RESOURCES; BIOMEDICAL APPLICATIONS; PERIODIC STRUCTURES; COLLOIDAL GELS AB Shape memory polymers (SMPs) are attractive materials due to their unique mechanical properties, including high deformation capacity and shape recovery. SMPs are easier to process, lightweight, and inexpensive compared to their metallic counterparts, shape memory alloys. However, SMPs are limited to relatively small form factors due to their low recovery stresses. Lightweight, micro-architected composite SMPs may overcome these size limitations and offer the ability to combine functional properties (e.g., electrical conductivity) with shape memory behavior. Fabrication of 3D SMP thermoset structures via traditional manufacturing methods is challenging, especially for designs that are composed of multiple materials within porous microarchitectures designed for specific shape change strategies, e.g. sequential shape recovery. We report thermoset SMP composite inks containing some materials from renewable resources that can be 3D printed into complex, multi-material architectures that exhibit programmable shape changes with temperature and time. Through addition of fiber-based fillers, we demonstrate printing of electrically conductive SMPs where multiple shape states may induce functional changes in a device and that shape changes can be actuated via heating of printed composites. The ability of SMPs to recover their original shapes will be advantageous for a broad range of applications, including medical, aerospace, and robotic devices. C1 [Rodriguez, Jennifer N.; Zhu, Cheng; Duoss, Eric B.; Wilson, Thomas S.; Spadaccini, Christopher M.; Lewicki, James P.] Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. RP Rodriguez, JN; Duoss, EB (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. EM rodriguez96@llnl.gov; duoss1@llnl.gov FU Lawrence Livermore National Laboratory under U.S. Department of Energy [DE-AC52-07NA27344]; Lawrence Livermore National Laboratory through LDRD award [14-SI-004, 15-ERD-030, LLNL-JRNL-680227] FX The authors would like to thank Peter Frankel and Galata Chemicals, for their interest in this research and generous samples of epoxidized soybean oil. The authors would like to thank Ward Small IV for his training and discussions in regards to dynamic mechanical thermal analysis and Patrick G. Campbell for his training and expertise in scanning electron microscopy. The authors would also like to thank Fang Qian for generously supplying CNFs. This work was supported by Lawrence Livermore National Laboratory under the auspices of the U.S. Department of Energy under Contract DE-AC52-07NA27344, through LDRD award 14-SI-004 and 15-ERD-030 with IM Release No: LLNL-JRNL-680227. NR 43 TC 1 Z9 1 U1 35 U2 35 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JUN 15 PY 2016 VL 6 AR 27933 DI 10.1038/srep27933 PG 10 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DY3FM UT WOS:000384976200001 PM 27301435 ER PT J AU Nandasiri, MI Liu, J McGrail, BP Jenks, J Schaef, HT Shutthanandan, V Nie, ZM Martin, PF Nune, SK AF Nandasiri, Manjula I. Liu, Jian McGrail, B. Peter Jenks, Jeromy Schaef, Herbert T. Shutthanandan, Vaithiyalingam Nie, Zimin Martin, Paul F. Nune, Satish K. TI Increased Thermal Conductivity in Metal-Organic Heat Carrier Nanofluids SO SCIENTIFIC REPORTS LA English DT Article ID MIL-101/GRAPHENE OXIDE COMPOSITES; GRAPHENE OXIDE; ADSORPTION PERFORMANCE; FRAMEWORK; ADSORBENTS; CAPACITY; MOF; GRO-AT-MIL-101; NANOPARTICLES; SEPARATION AB Metal-organic heat carriers (MOHCs) are recently developed nanofluids containing metal-organic framework (MOF) nanoparticles dispersed in various base fluids including refrigerants (R245Fa) and methanol. Here, we report the synthesis and characterization of MOHCs containing nanoMIL-101(Cr) and graphene oxide (GO) in an effort to improve the thermo-physical properties of various base fluids. MOHC/GO nanocomposites showed enhanced surface area, porosity, and nitrogen adsorption compared with the intrinsic nanoMIL-101(Cr) and the properties depended on the amount of GO added. MIL-101(Cr)/GO in methanol exhibited a significant increase in the thermal conductivity (by approximately 50%) relative to that of the intrinsic nanoMIL-101(Cr) in methanol. The thermal conductivity of the base fluid (methanol) was increased by about 20%. The increase in the thermal conductivity of nanoMIL-101(Cr) MOHCs due to GO functionalization is explained using a classical Maxwell model. C1 [Nandasiri, Manjula I.; Shutthanandan, Vaithiyalingam] Pacific Northwest Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Liu, Jian; McGrail, B. Peter; Jenks, Jeromy; Nie, Zimin; Martin, Paul F.; Nune, Satish K.] Pacific Northwest Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. [Schaef, Herbert T.] Pacific Northwest Natl Lab, Fundamental Chem Sci Directorate, Richland, WA 99352 USA. RP Nune, SK (reprint author), Pacific Northwest Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. EM satish.nune@pnnl.gov RI Liu, Jian/D-3393-2009 OI Liu, Jian/0000-0001-5329-7408 FU U.S. Department of Energy (DOE), Office of Energy Efficiency and Renewable Energy Geothermal Technologies Program [DE-PS36-09GO99017]; U.S. Department of Energy by Battelle Memorial Institute [DE-AC05-76RL01830]; Department of Energy's Office of Biological and Environmental Research FX This work was supported by the U.S. Department of Energy (DOE), Office of Energy Efficiency and Renewable Energy Geothermal Technologies Program under Funding Opportunity Announcement DE-PS36-09GO99017. The Pacific Northwest National Laboratory is a multi-programme national laboratory operated for the U.S. Department of Energy by Battelle Memorial Institute under Contract DE-AC05-76RL01830. XPS and SEM characterizations were performed at EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research, located at PNNL. NR 52 TC 0 Z9 0 U1 19 U2 19 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JUN 15 PY 2016 VL 6 AR 27805 DI 10.1038/srep27805 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DX8DE UT WOS:000384617500001 PM 27302196 ER PT J AU Shanavas, KV Lindsay, L Parker, DS AF Shanavas, K. V. Lindsay, L. Parker, D. S. TI Electronic structure and electron-phonon coupling in TiH2 SO SCIENTIFIC REPORTS LA English DT Article ID AB-INITIO; SUPERCONDUCTIVITY; HYDROGEN; HYDRIDES; SYSTEM; TEMPERATURE; ZIRCONIUM; PRESSURE; METALS AB Calculations using first principles methods and strong coupling theory are carried out to understand the electronic structure and superconductivity in cubic and tetragonal TiH2. A large electronic density of states at the Fermi level in the cubic phase arises from Ti-t(2g) states and leads to a structural instability towards tetragonal distortion at low temperatures. However, constraining the in-plane lattice constants diminishes the energy gain associated with the tetragonal distortion, allowing the cubic phase to be stable at low temperatures. Calculated phonon dispersions show decoupled acoustic and optic modes arising from Ti and H vibrations, respectively, and frequencies of optic modes to be rather high. The cubic phase has a large electron-phonon coupling parameter lambda and critical temperature of several K. Contribution of the hydrogen sublattice to lambda is found to be small in this material, which we understand from strong coupling theory to be due to the small H-s DOS at the Fermi level and high energy of hydrogen modes at the tetrahedral sites. C1 [Shanavas, K. V.; Lindsay, L.; Parker, D. S.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Shanavas, KV (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. EM shanavaskv@gmail.com RI Lindsay, Lucas/C-9221-2012 OI Lindsay, Lucas/0000-0001-9645-7993 FU US Department of Energy, Basic Energy Sciences, Office of Science, Materials Sciences and Engineering Division FX This research was supported by the US Department of Energy, Basic Energy Sciences, Office of Science, Materials Sciences and Engineering Division. NR 31 TC 0 Z9 0 U1 16 U2 16 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JUN 15 PY 2016 VL 6 AR 28102 DI 10.1038/srep28102 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DX7ZI UT WOS:000384607500001 PM 27302645 ER PT J AU Zhou, GN Zhu, WX Shen, H Li, Y Zhang, AF Tamura, N Chen, K AF Zhou, Guangni Zhu, Wenxin Shen, Hao Li, Yao Zhang, Anfeng Tamura, Nobumichi Chen, Kai TI Real-time microstructure imaging by Laue microdiffraction: A sample application in laser 3D printed Ni-based superalloys SO SCIENTIFIC REPORTS LA English DT Article ID SINGLE-CRYSTAL SUPERALLOY; DIFFRACTION PATTERNS; CARBON ADDITIONS; MC CARBIDE; SYNCHROTRON; FRACTURE; QUARTZ AB Synchrotron-based Laue microdiffraction has been widely applied to characterize the local crystal structure, orientation, and defects of inhomogeneous polycrystalline solids by raster scanning them under a micro/nano focused polychromatic X-ray probe. In a typical experiment, a large number of Laue diffraction patterns are collected, requiring novel data reduction and analysis approaches, especially for researchers who do not have access to fast parallel computing capabilities. In this article, a novel approach is developed by plotting the distributions of the average recorded intensity and the average filtered intensity of the Laue patterns. Visualization of the characteristic microstructural features is realized in real time during data collection. As an example, this method is applied to image key features such as microcracks, carbides, heat affected zone, and dendrites in a laser assisted 3D printed Ni-based superalloy, at a speed much faster than data collection. Such analytical approach remains valid for a wide range of crystalline solids, and therefore extends the application range of the Laue microdiffraction technique to problems where real-time decision-making during experiment is crucial (for instance time-resolved non-reversible experiments). C1 [Zhou, Guangni; Zhu, Wenxin; Shen, Hao; Li, Yao; Chen, Kai] Xi An Jiao Tong Univ, State Key Lab Mech Behav Mat, Ctr Advancing Mat Performance Nanoscale CAMP Nano, Xian 710049, Shaanxi, Peoples R China. [Zhang, Anfeng] Xi An Jiao Tong Univ, State Key Lab Mfg Syst Engn, Xian 710049, Shaanxi, Peoples R China. [Tamura, Nobumichi] Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Chen, K (reprint author), Xi An Jiao Tong Univ, State Key Lab Mech Behav Mat, Ctr Advancing Mat Performance Nanoscale CAMP Nano, Xian 710049, Shaanxi, Peoples R China. EM kchenlbl@gmail.com RI xjtu, campnano/Q-1904-2015 FU National Natural Science Foundation of China [51302207, 51275392, 11132006]; National Basic Research Program of China ("973" Program) [2015CB057400]; Fundamental Research Funds for the Central Universities [2015gjhz03]; Collaborative Innovation Center of High-End Manufacturing Equipment; International Joint Laboratory for Micro/Nano Manufacturing and Measurement Technologies; National Young 1000 Talents Program of China; Office of Science, Office of Basic Energy Sciences, Materials Science Division, of the U.S. Department of Energy at LBNL [DE-AC02-05CH11231] FX This work is supported by the National Natural Science Foundation of China (Grant No. 51302207, 51275392, 11132006), the National Basic Research Program of China ("973" Program) (Grant No. 2015CB057400), and the Fundamental Research Funds for the Central Universities (Grant No. 2015gjhz03). We also appreciate the support from the Collaborative Innovation Center of High-End Manufacturing Equipment and the International Joint Laboratory for Micro/Nano Manufacturing and Measurement Technologies. KC is supported by the National Young 1000 Talents Program of China. The ALS is supported by the Director, Office of Science, Office of Basic Energy Sciences, Materials Science Division, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231 at LBNL. NR 39 TC 1 Z9 1 U1 16 U2 16 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JUN 15 PY 2016 VL 6 AR 28144 DI 10.1038/srep28144 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DX7ZW UT WOS:000384608900001 PM 27302087 ER PT J AU McLing, TL Smith, RP Smith, RW Blackwell, DD Roback, RC Sondrup, AJ AF McLing, Travis L. Smith, Richard P. Smith, Robert W. Blackwell, David D. Roback, Robert C. Sondrup, Andrus J. TI Wellbore and groundwater temperature distribution eastern Snake River Plain, Idaho: Implications for groundwater flow and geothermal potential SO JOURNAL OF VOLCANOLOGY AND GEOTHERMAL RESEARCH LA English DT Article DE Eastern Snake River Plain; Thermal groundwater tracer; Groundwater flow; Temperature distribution ID RANGE VOLCANIC ARC; HEAT-FLOW; SUBSURFACE TEMPERATURES; TECTONIC IMPLICATIONS; MOUNTAINOUS TERRAIN; AQUIFER; SYSTEMS; PATTERNS; RATES; BASALT AB A map of groundwater temperatures from the Eastern Snake River Plain (ESRP) regional aquifer can be used to identify and interpret important features of the aquifer, including aquifer flow direction, aquifer thickness, and potential geothermal anomalies. The ESRP is an area of high heat flow, yet most of this thermal energy fails to reach the surface, due to the heat being swept downgradient by the aquifer to the major spring complexes near Thousand Springs, ID, a distance of 300 km Nine deep boreholes that fully penetrate the regional aquifer display three common features: (1) high thermal gradients beneath the aquifer, corresponding to high conductive heat flow in low-permeability hydrothermally-altered rocks; (2) isothermal temperature profiles within the aquifer, characteristic of an actively flowing groundwater; and (3) moderate thermal gradients in the vadose zone with values that indicate that over half of the geothermal heat flow is removed by advective transport in the regional aquifer system. This study utilized temperature data from 250 ESRP aquifer wells to evaluate regional aquifer flow direction, aquifer thickness, and potential geothermal anomalies. Because the thermal gradients are typically low in the aquifer, any measurement of groundwater temperature is a reasonable estimate of temperature throughout the aquifer thickness, allowing the construction of a regional aquifer temperature map for the ESRP. Mapped temperatures are used to identify cold thermal plumes associated with recharge from tributary valleys and adjacent uplands, and warm zones associated with geothermal input to the aquifer. Warm zones in the aquifer can have various causes, including local circulation of groundwater through the deep conductively dominated region, slow groundwater movement in low-permeability regions, or localized heat flow from deeper thermal features. Published by Elsevier B.V. C1 [McLing, Travis L.; Sondrup, Andrus J.] Idaho Natl Lab, POB 1625, Idaho Falls, ID 83415 USA. [McLing, Travis L.] Ctr Adv Energy Studies, 995 Univ Blvd, Idaho Falls, ID 83401 USA. [Smith, Richard P.] Smith Geol & Photog Serv LLC, Nathrop, CO 81236 USA. [Smith, Robert W.; Blackwell, David D.] Univ Idaho, Moscow, ID 83844 USA. [Roback, Robert C.] Los Alamos Natl Lab, Earth & Environm Sci Div, Los Alamos, NM 87545 USA. RP McLing, TL (reprint author), Idaho Natl Lab, POB 1625, Idaho Falls, ID 83415 USA. EM travis.mcling@inl.gov OI Roback, Robert/0000-0003-2748-1580 NR 59 TC 1 Z9 1 U1 5 U2 7 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0377-0273 EI 1872-6097 J9 J VOLCANOL GEOTH RES JI J. Volcanol. Geotherm. Res. PD JUN 15 PY 2016 VL 320 BP 144 EP 155 DI 10.1016/j.jvolgeores.2016.04.006 PG 12 WC Geosciences, Multidisciplinary SC Geology GA DR7JC UT WOS:000380074900014 ER PT J AU Bollani, M Giliberti, V Sakat, E Baldassarre, L Celebrano, M Frigerio, J Isella, G Finazzi, M Melli, M Weber-Bargioni, A Cabrini, S Biagioni, P Ortolani, M AF Bollani, M. Giliberti, V. Sakat, E. Baldassarre, L. Celebrano, M. Frigerio, J. Isella, G. Finazzi, M. Melli, M. Weber-Bargioni, A. Cabrini, S. Biagioni, P. Ortolani, M. TI Photoluminescence emission from a nanofabricated scanning probe tip made of epitaxial germanium SO MICROELECTRONIC ENGINEERING LA English DT Article; Proceedings Paper CT 6th Micro and Nano Conference CY OCT 04-07, 2015 CL GREECE DE Scanning probe tip; Photoluminescence; Nano-optics; Focused ion beam ID FIELD OPTICAL MICROSCOPY; RESOLUTION LIMIT; LIGHT-SOURCE; SILICON AB We discuss a new type of nanoscale photon source constituted by a micro-pyramid made of epitaxial semiconductor material (Ge) attached to a silicon cantilever optimized for Atomic Force Microscopy and shaped by means of low-current Focused Ion Beam (FIB) milling. The optical characterization of these tips demonstrates sizeable photoluminescence emission at the direct energy gap of Ge (1550 nm). We have checked by independent measurements on the nano-patterned epitaxial material prior to the tip shaping process that the photoluminescence yield is not significantly affected by FIB milling, indicating that the optical properties of the material in this wavelength range are preserved. We envisage an application of this tool as a scanning probe in apertureless scanning near-field optical microscopy. (C) 2016 Elsevier B.V. All rights reserved. C1 [Bollani, M.] IFN CNR, LNESS Lab, I-22100 Como, Italy. [Giliberti, V.; Baldassarre, L.; Ortolani, M.] Sapienza Univ Rome, Dipartimento Fis, I-00185 Rome, Italy. [Sakat, E.; Celebrano, M.; Finazzi, M.; Biagioni, P.] Politecn Milan, Dipartimento Fis, I-20133 Milan, Italy. [Baldassarre, L.] Italian Inst Technol, Ctr Life & Nano Sci, I-00185 Rome, Italy. [Frigerio, J.; Isella, G.] Politecn Milan, Dipartimento Fis, LNESS, I-22100 Como, Italy. [Melli, M.; Weber-Bargioni, A.; Cabrini, S.] Lawrence Berkeley Natl Labs, Mol Foundry, Berkeley, CA 94720 USA. RP Bollani, M (reprint author), IFN CNR, LNESS Lab, I-22100 Como, Italy. EM monica.bollani@ifn.cnr.it RI Biagioni, Paolo/A-9940-2011; Celebrano, Michele/D-6503-2011; Isella, Giovanni/A-7305-2008; Bollani, Monica/D-7630-2013; Baldassarre, Leonetta/H-4637-2013; OI Biagioni, Paolo/0000-0003-4272-7040; Celebrano, Michele/0000-0003-3336-3580; Isella, Giovanni/0000-0001-5951-7440; Bollani, Monica/0000-0002-0078-5085; Baldassarre, Leonetta/0000-0003-2217-0564; ortolani, michele/0000-0002-7203-5355 NR 20 TC 0 Z9 0 U1 7 U2 9 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-9317 EI 1873-5568 J9 MICROELECTRON ENG JI Microelectron. Eng. PD JUN 15 PY 2016 VL 159 SI SI BP 164 EP 168 DI 10.1016/j.mee.2016.03.047 PG 5 WC Engineering, Electrical & Electronic; Nanoscience & Nanotechnology; Optics; Physics, Applied SC Engineering; Science & Technology - Other Topics; Optics; Physics GA DQ1LQ UT WOS:000378962900035 ER PT J AU Zhao, YX Anderson, NC Ratzloff, MW Mulder, DW Zhu, K Turner, JA Neale, NR King, PW Branz, HM AF Zhao, Yixin Anderson, Nicholas C. Ratzloff, Michael W. Mulder, David W. Zhu, Kai Turner, John A. Neale, Nathan R. King, Paul W. Branz, Howard M. TI Proton Reduction Using a Hydrogenase-Modified Nanoporous Black Silicon Photoelectrode SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE photoelectrochemical water splitting; hydrogen production; hydrogenase; silicon photoelectrode; bio-assisted; black silicon ID ATOMIC LAYER DEPOSITION; H-2 PRODUCTION; EVOLUTION REACTION; PHOSPHIDE NANOPARTICLES; MOS2 NANOPARTICLES; OXIDATION; CATALYSTS; ELECTROCATALYSTS; ENZYMES; PHOTOCATHODES AB Metalloenzymes featuring earth-abundant metal-based cores exhibit rates for catalytic processes such as hydrogen evolution comparable to those of noble metals. Realizing these superb catalytic properties in artificial systems is challenging owing to the difficulty of effectively interfacing metalloenzymes with an electrode surface in a manner that supports efficient charge-transfer. Here, we demonstrate that a nanoporous black silicon (b-Si) photocathode provides a unique interface for binding an adsorbed [FeFe]-hydrogenase enzyme ([FeFe]-H(2)ase). The resulting [FeFe]-H(2)ase/b-Si photoelectrode displays a 280 mV more positive onset potential for hydrogen generation than bare b-Si without hydrogenase, similar to that observed for a b-Si/Pt photoelectrode at the same light intensity. Additionally, we show that this H(2)ase/b-Si electrode exhibits a turnover frequency of >= 1300 s(-1) and a turnover number above 10(7) and sustains current densities of at least 1 mA/cm(2) based on the actual surface area of the electrode (not the smaller projected geometric area), orders of magnitude greater than that observed for previous enzyme-catalyzed electrodes. While the long-term stability of hydrogenase on the b-Si surface remains too low for practical applications, this work extends the proof-of-concept that biologically derived metalloenzymes can be interfaced with inorganic substrates to support technologically relevant current densities. C1 [Zhao, Yixin; Anderson, Nicholas C.; Ratzloff, Michael W.; Mulder, David W.; Zhu, Kai; Turner, John A.; Neale, Nathan R.; King, Paul W.; Branz, Howard M.] Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. [Zhao, Yixin] Shanghai Jiao Tong Univ, 800 Dongchuan Rd, Shanghai 200240, Peoples R China. RP Neale, NR; King, PW; Branz, HM (reprint author), Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. EM nathan.neale@nrel.gov; paul.king@nrel.gov; howard@branztechnologypartners.com RI King, Paul/D-9979-2011; Zhao, Yixin/D-2949-2012; OI King, Paul/0000-0001-5039-654X; Anderson, Nicholas/0000-0001-8161-5303 FU Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy [DEAC36-08GO28308] FX This work was supported by the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy, under Contract No. DEAC36-08GO28308. NR 51 TC 1 Z9 1 U1 9 U2 32 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD JUN 15 PY 2016 VL 8 IS 23 BP 14481 EP 14487 DI 10.1021/acsami.6b00189 PG 7 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DP0QT UT WOS:000378195000022 PM 27219350 ER PT J AU Yen, HJ Liang, PW Chueh, CC Yang, ZB Jen, AKY Wang, HL AF Yen, Hung-Ju Liang, Po-Wei Chueh, Chu-Chen Yang, Zhibin Jen, Alex K-Y. Wang, Hsing-Lin TI Large Grained Perovskite Solar Cells Derived from Single-Crystal Perovskite Powders with Enhanced Ambient Stability SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE perovskite; single crystal; large grain; ambient stability; solar cell ID ORGANOMETAL HALIDE PEROVSKITES; CH3NH3PBX3 X; TRIHALIDE; DIFFUSION; LENGTHS; GROWTH; LAYERS; BR AB In this study, we demonstrate the large grained perovskite solar cells prepared from precursor solution comprising Single-crystal perovskite powders for the first time. The resultant large grained perovskite thin film possesses a negligible physical (structural) gap between each large grain and is highly crystalline as evidenced by its fan-shaped birefringence observed under polarized light, which is very different from the thin film prepared from the typical precursor route (MAI + PbI2). C1 [Yen, Hung-Ju; Wang, Hsing-Lin] Los Alamos Natl Lab, Div Chem, Phys Chem & Appl Spect C PCS, POB 1663, Los Alamos, NM 87545 USA. [Liang, Po-Wei; Chueh, Chu-Chen; Yang, Zhibin; Jen, Alex K-Y.] Univ Washington, Dept Mat Sci & Engn, Seattle, WA 98195 USA. [Jen, Alex K-Y.] Univ Washington, Dept Chem, Seattle, WA 98195 USA. RP Wang, HL (reprint author), Los Alamos Natl Lab, Div Chem, Phys Chem & Appl Spect C PCS, POB 1663, Los Alamos, NM 87545 USA.; Jen, AKY (reprint author), Univ Washington, Dept Mat Sci & Engn, Seattle, WA 98195 USA.; Jen, AKY (reprint author), Univ Washington, Dept Chem, Seattle, WA 98195 USA. EM ajen@u.washington.edu; hwang@lanl.gov RI Yang, Zhibin/F-6212-2015; OI Yang, Zhibin/0000-0003-4036-9446; Yen, Hung-Ju/0000-0002-6316-9124 FU Laboratory Directed Research and Development program under U.S. Department of Energy; J. R. Oppenheimer Fellowship; Office of Naval Research [N00014-14-1-0246]; Asian Office of Aerospace RD [FA2386-11-1-4072]; Department of Energy SunShot [DE-EE0006710]; Boeing-Johnson Foundation FX H.-J.Y. and H.-L.W. thank the financial support by the Laboratory Directed Research and Development program under the auspices of the U.S. Department of Energy. H.J.Y. thanks the J. R. Oppenheimer Fellowship for supporting the materials synthesis and characterization. A.K.-Y.J. thanks the financial support by the Office of Naval Research (N00014-14-1-0246), the Asian Office of Aerospace R&D (FA2386-11-1-4072), the Department of Energy SunShot (DE-EE0006710), and the Boeing-Johnson Foundation. NR 38 TC 8 Z9 8 U1 23 U2 88 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD JUN 15 PY 2016 VL 8 IS 23 BP 14513 EP 14520 DI 10.1021/acsami.6b02169 PG 8 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DP0QT UT WOS:000378195000026 PM 27224963 ER PT J AU Yang, N Shi, YU Schweiger, S Strelcov, E Belianinov, A Foglietti, V Orgiani, P Balestrino, G Kalinin, SV Rupp, JLM Aruta, C AF Yang, Nan Shi, Yanuo Schweiger, Sebastian Strelcov, Evgheni Belianinov, Alex Foglietti, Vittorio Orgiani, Pasquale Balestrino, Giuseppe Kalinin, Sergei V. Rupp, Jennifer L. M. Aruta, Carmela TI Role of Associated Defects in Oxygen Ion Conduction and Surface Exchange Reaction for Epitaxial Samaria-Doped Ceria Thin Films as Catalytic Coatings SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE doped ceria; epitaxial thin films; defect associations; Raman; electrochemical strain microscopy ID OXIDE FUEL-CELLS; STRUCTURAL-CHARACTERIZATION; NONSTOICHIOMETRIC CERIA; ENERGY-CONVERSION; SOLID-SOLUTIONS; CO2 REDUCTION; CEO2; TRANSPORT; ELECTROLYTE; MEMBRANES AB Samaria-doped ceria (SDC) thin films are particularly important for energy and electronic applications such as microsolid oxide fuel cells, electrolyzers, sensors, and memristors. In this paper, we report a comparative study investigating ionic conductivity and surface reactions for well-grown epitaxial SDC films varying the samaria doping concentration. With increasing doping above 20 mol % of samaria, an enhancement in the defect association is observed by Raman spectroscopy. The role of such associated defects on the films oxygen ion transport and exchange is investigated by electrochemical impedance spectroscopy and electrochemical strain microscopy (ESM). The measurements reveal that the ionic transport has a sharp maximum in ionic conductivity and drops in its activation energy down to 0.6 eV for 20 mol % doping. Increasing the doping concentration further up to 40 mol %, it raises the activation energy substantially by a factor of 2. We ascribe the sluggish transport kinetics to the "bulk" ionic-near ordering in case of the heavily doped epitaxial films. Analysis of the ESM first-order reversal curve measurements indicates that these associated defects may have a beneficial role by lowering-the activation of the oxygen exchange "surface" reaction for heavily doped 40 mol % of samaria. In a model experiment, through a solid solution series of samaria doped ceria epitaxial films, we reveal that the occurrence of associated defects in the bulk affects: the surface charging state of the SDC films to increase the exchange rates. The implication of these findings is the design of coatings with tuned oxygen surface exchange by controlling the bulk associated clusters for future electrocatalytic applications. C1 [Yang, Nan; Foglietti, Vittorio; Balestrino, Giuseppe; Aruta, Carmela] Univ Roma Tor Vergata, Natl Res Council CNR SPIN, I-00133 Rome, Italy. [Yang, Nan; Foglietti, Vittorio; Balestrino, Giuseppe] Univ Roma Tor Vergata, Dept DICII, I-00133 Rome, Italy. [Shi, Yanuo; Schweiger, Sebastian; Rupp, Jennifer L. M.] ETH, Electrochem Mat, CH-8093 Zurich, Switzerland. [Strelcov, Evgheni; Belianinov, Alex; Kalinin, Sergei V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Orgiani, Pasquale] Univ Salerno, Natl Res Council CNR SPIN, I-84084 Salerno, Italy. [Orgiani, Pasquale] Natl Res Council CNR IOM, TASC Natl Lab, I-34149 Trieste, Italy. RP Aruta, C (reprint author), Univ Roma Tor Vergata, Natl Res Council CNR SPIN, I-00133 Rome, Italy. EM carmela.aruta@spin.cnr.it RI Foglietti, Vittorio/J-7052-2012; Aruta, Carmela/L-2957-2015; Orgiani, Pasquale/E-7146-2013 OI Foglietti, Vittorio/0000-0002-9588-5379; Aruta, Carmela/0000-0002-6917-6667; Orgiani, Pasquale/0000-0002-1082-9651 FU CNR-Short-term Mobility program; Italian MIUR FIRB project [RBAP115AYN]; PRIN project OXIDE; Swiss National Science Foundation [147190, 155986, 138914] FX Author N.Y. received funding from CNR-Short-term Mobility program 2015. Authors N.Y., P.O., G.B. and C.A. received funding from Italian MIUR FIRB project RBAP115AYN and PRIN project 2010-2011 OXIDE. Authors Y.S., S.S. and J.L.M.R. received funding from Swiss National Science Foundation project numbers 147190, 155986 and 138914. NR 52 TC 4 Z9 4 U1 19 U2 29 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD JUN 15 PY 2016 VL 8 IS 23 BP 14613 EP 14621 DI 10.1021/acsami.6b03909 PG 9 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DP0QT UT WOS:000378195000040 PM 27192540 ER PT J AU Gao, R Dong, YQ Xu, H Zhou, H Yuan, YK Gopalan, V Gao, C Fong, DD Chen, ZH Luo, ZL Martin, LW AF Gao, Ran Dong, Yongqi Xu, Han Zhou, Hua Yuan, Yakun Gopalan, Venkatraman Gao, Chen Fong, Dillon D. Chen, Zuhuang Luo, Zhenlin Martin, Lane W. TI Interfacial Octahedral Rotation Mismatch Control of the Symmetry and Properties of SrRuO3 SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE SrRuO3; epitaxial strain; octahedral rotation; interfacial engineering; crystal symmetry ID THIN-FILMS; OXIDE HETEROSTRUCTURES; PEROVSKITES; HETEROINTERFACE; DISTORTIONS AB Epitaxial Strain can be used to tune the properties of complex oxides with perovskite structure. Beyond just lattice mismatch, the use of octahedral rotation mismatch at heterointerfaces could also provide an effective route to manipulate material properties. Here, we examine the evolution of the structural motif (i.e., lattice parameters, symmetry, and octahedral: rotations) of SrRuO3 films grown on substrates engineered to have the same lattice parameters, but different octahedral rotations. SrRuO3 films grown on SrTiO3 (001) (no octahedral rotations) and GdScO3 buffered SrTiO3 (001) (with octahedral rotations) substrates are found to exhibit monoclinic and tetragonal symmetry, respectively. Electrical transport and magnetic measurements reveal that the tetragonal films exhibit higher resistivity, lower magnetic Curie temperatures) and more isotropic magnetism as compared to those with monoclinic structure. Synchrotron-based quantification Of the octahedral rotation network reveals that the tilting pattern in both film variants is the same (albeit with slightly different magnitudes of in-plane rotation angles): The abnormal rotation pattern observed in tetragonal SrRuO3 indicates a possible decoupling between the internal octahedral rotation and lattice symmetry, which could provide new opportunities to engineer thin-film structure and properties. C1 [Gao, Ran; Chen, Zuhuang; Martin, Lane W.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Dong, Yongqi; Xu, Han; Gao, Chen; Luo, Zhenlin] Univ Sci & Technol China, Natl Synchrotron Radiat Lab, Hefei 230026, Anhui, Peoples R China. [Dong, Yongqi; Xu, Han; Gao, Chen; Luo, Zhenlin] Univ Sci & Technol China, CAS Key Lab Mat Energy Convers, Hefei 230026, Anhui, Peoples R China. [Zhou, Hua] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. [Yuan, Yakun; Gopalan, Venkatraman] Penn State Univ, Dept Mat Sci & Engn, State Coll, PA 16802 USA. [Fong, Dillon D.] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. [Chen, Zuhuang; Martin, Lane W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Chen, ZH; Martin, LW (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA.; Chen, ZH; Martin, LW (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM zuhuang@berkeley.edu; lwmartin@berkeley.edu RI Martin, Lane/H-2409-2011; Chen, Zuhuang/E-7131-2011 OI Martin, Lane/0000-0003-1889-2513; Chen, Zuhuang/0000-0003-1912-6490 FU Air Force Office of Scientific Research [FA9550-12-1-0471]; Advanced Photon Source [12-ID-D]; Shanghai Synchrotron Radiation Facility [14B]; National Natural Science Foundation of China [11374010, 11434009]; DOE Office of Science by Argonne National Laboratory [DE-AC02-06CH11357]; Penn State MRSEC Center for Nanoscale Science [DMR-1420620]; U.S. Department of Energy Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; Laboratory Directed Research and Development Program of Lawrence Berkeley National Laboratory under U.S. Department of Energy [DE-AC02-05CH11231]; U.S. Department of Energy, Office of Basic Energy Science [DE-SC0012375] FX R. Gao acknowledges support from the Air Force Office of Scientific Research under Grant FA9550-12-1-0471. H.X, Z.L.L., and C. Gao acknowledge the support from 12-ID-D at the Advanced Photon Source and 14B at Shanghai Synchrotron Radiation Facility. Z.L.L. also acknowledges the support from the National Natural Science Foundation of China (Grant Nos. 11374010 and 11434009). H.Z. acknowledges support from the resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. Y.Y. and V.G. gratefully acknowledge support from the Penn State MRSEC Center for Nanoscale Science, Grant DMR-1420620. D.D.F. acknowledges support from the U.S. Department of Energy Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. Z.C. acknowledges support from the Laboratory Directed Research and Development Program of Lawrence Berkeley National Laboratory under U.S. Department of Energy Contract No. DE-AC02-05CH11231 for the development of the SrRuO3 films. L.W.M. acknowledges support from the U.S. Department of Energy, Office of Basic Energy Science under Contract No. DE-SC0012375 for the development of metastable SrRuO3 structures. NR 44 TC 2 Z9 2 U1 21 U2 47 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD JUN 15 PY 2016 VL 8 IS 23 BP 14871 EP 14878 DI 10.1021/acsami.6b02864 PG 8 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DP0QT UT WOS:000378195000069 PM 27219026 ER PT J AU Boys, CA Robinson, W Miller, B Pflugrath, B Baumgartner, LJ Navarro, A Brown, R Deng, ZQ AF Boys, Craig A. Robinson, Wayne Miller, Brett Pflugrath, Brett Baumgartner, Lee J. Navarro, Anna Brown, Richard Deng, Zhiqun TI How low can they go when going with the flow? Tolerance of egg and larval fishes to rapid decompression SO BIOLOGY OPEN LA English DT Article DE Barotrauma; Hydropower; Larval drift; Murray-Darling basin; Physoclistous; Piecewise regression ID MACCULLOCHELLA-PEELII-PEELII; SWIM BLADDER INFLATION; HYDRO-TURBINE PASSAGE; DARLING RIVER SYSTEM; HYDROTURBINE PASSAGE; STRIPED BASS; GOLDEN PERCH; GAS BLADDER; BAROTRAUMA; MORTALITY AB Egg and larval fish that drift downstream are likely to encounter river infrastructure and consequently rapid decompression, which may result in significant injury. Pressure-related injury (or barotrauma) has been shown in juvenile fishes when pressure falls sufficiently below that at which the fish has acclimated. There is a presumption that eggs and larvae may be at least as, if not more, susceptible to barotrauma injury because they are far less-developed and more fragile than juveniles, but studies to date report inconsistent results and none have considered the relationship between pressure change and barotrauma over a sufficiently broad range of pressure changes to enable tolerances to be properly determined. To address this, we exposed eggs and larvae of three physoclistic species to rapid decompression in a barometric chamber over a broad range of discrete pressure changes. Eggs, but not larvae, were unaffected by all levels of decompression tested. At exposure pressures below similar to 40 kPa, or similar to 40% of surface pressure, swim bladder deflation occurred in all species and internal haemorrhage was observed in one species. None of these injuries killed the fish within 24 h, but subsequent mortality cannot be excluded. Consequently, if larval drift is expected where river infrastructure is present, adopting design or operational features which maintain exposure pressures at 40% or more of the pressure to which drifting larvae are acclimated may afford greater protection for resident fishes. C1 [Boys, Craig A.; Baumgartner, Lee J.] Port Stephens Fisheries Inst, New South Wales Dept Primary Ind, Taylors Beach Rd, Taylors Beach, NSW 2316, Australia. [Robinson, Wayne; Baumgartner, Lee J.; Navarro, Anna] Charles Sturt Univ, Inst Land Water & Soc, Elizabeth Mitchell Dr Thurgoona, Albury, NSW 2640, Australia. [Robinson, Wayne; Baumgartner, Lee J.] Narrandera Fisheries Ctr, New South Wales Dept Primary Ind, 64 Buckingbong Rd Narrandera, Narrandera, NSW 2700, Australia. [Pflugrath, Brett] Univ New S Wales, Water Res Lab, 110 King St Manly Vale, Sydney, NSW 2093, Australia. [Brown, Richard; Deng, Zhiqun] Pacific NW Natl Lab, Richland, WA 99354 USA. RP Boys, CA (reprint author), Port Stephens Fisheries Inst, New South Wales Dept Primary Ind, Taylors Beach Rd, Taylors Beach, NSW 2316, Australia. EM craig.boys@dpi.nsw.gov.au RI Deng, Daniel/A-9536-2011; OI Deng, Daniel/0000-0002-8300-8766; Navarro Cuenca, Anna/0000-0003-3762-4135 FU New South Wales Department of Primary Industries (NSW DPI); Australian Renewable Energy Agency (ARENA) Emerging Renewables Program FX This project was funded in part by New South Wales Department of Primary Industries (NSW DPI) and grants provided by the Australian Renewable Energy Agency (ARENA) Emerging Renewables Program (devolved through Waratah Power) and the Australian Centre for International Agricultural Research (ACIAR). NR 47 TC 0 Z9 0 U1 4 U2 12 PU COMPANY OF BIOLOGISTS LTD PI CAMBRIDGE PA BIDDER BUILDING CAMBRIDGE COMMERCIAL PARK COWLEY RD, CAMBRIDGE CB4 4DL, CAMBS, ENGLAND SN 2046-6390 J9 BIOL OPEN JI Biol. Open PD JUN 15 PY 2016 VL 5 IS 6 BP 786 EP 793 DI 10.1242/bio.017491 PG 8 WC Biology SC Life Sciences & Biomedicine - Other Topics GA DO9LZ UT WOS:000378109400014 PM 27230649 ER PT J AU Elder, T Berstis, L Beckham, GT Crowley, MF AF Elder, Thomas Berstis, Laura Beckham, Gregg T. Crowley, Michael F. TI Coupling and Reactions of 5-Hydroxyconiferyl Alcohol in Lignin Formation SO JOURNAL OF AGRICULTURAL AND FOOD CHEMISTRY LA English DT Article DE 5-hydroxyconiferyl alcohol; coniferyl alcohol; lignin; benzodioxane; stereochemistry ID BOND-DISSOCIATION ENTHALPIES; PHENETHYL PHENYL ETHER; DENSITY-FUNCTIONAL THEORY; MODEL COMPOUNDS; ALPHA/BETA-SELECTIVITIES; COMPUTATIONAL PREDICTION; PYROLYSIS MECHANISM; BETA-O-4; POLYMERIZATION; BIOSYNTHESIS AB The catechol alcohols, caffeyl and 5-hydroxyconiferyl alcohol, may be incorporated into lignin either naturally or through genetic manipulation. Due to the presence of o-OH groups, these compounds form benzodioxanes, a departure from the interunit connections found in lignins derived from the cinnamyl alcohols. In nature, lignins composed of caffeyl and 5-hydroxyconiferyl alcohol are linear homopolymers and, as such, may have properties that make them amenable for use in value-added products, such as lignin-based carbon fibers. In the current work, results from density functional theory calculations for the reactions of 5-hydroxyconiferyl alcohol, taking stereochemistry into account, are reported. Dehydrogenation and quinone methide formation are found to be thermodynamically favored for 5-hydroxyconiferyl alcohol, over coniferyl alcohol. The comparative energetics of the rearomatization reactions suggest that the formation of the benzodioxane linkage is under kinetic control. Ring-opening reactions of the benzodioxane groups show that the bond dissociation enthalpy of the alpha-O cleavage reaction is lower than that of the beta-O reaction. The catechol lignins represent a novel form of the polymer that may offer new opportunities for bioproducts and genetic targets. C1 [Elder, Thomas] Forest Serv, USDA, Southern Res Stn, 521 Devall Dr, Auburn, AL 36849 USA. [Berstis, Laura; Beckham, Gregg T.] Natl Renewable Energy Lab, Nat Bioenergy Ctr, 15013 Denver West Pkwy, Golden, CO 80401 USA. [Crowley, Michael F.] Natl Renewable Energy Lab, Biosci Ctr, 15013 Denver West Pkwy, Golden, CO 80401 USA. RP Elder, T (reprint author), Forest Serv, USDA, Southern Res Stn, 521 Devall Dr, Auburn, AL 36849 USA. EM telder@fs.fed.us FU US Department of Energy, Bioenergy Technologies Office FX L.B., G.T.B., and M.F.C. acknowledge funding from the US Department of Energy, Bioenergy Technologies Office. NR 41 TC 0 Z9 0 U1 7 U2 10 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0021-8561 EI 1520-5118 J9 J AGR FOOD CHEM JI J. Agric. Food Chem. PD JUN 15 PY 2016 VL 64 IS 23 BP 4742 EP 4750 DI 10.1021/acs.jafc.6b02234 PG 9 WC Agriculture, Multidisciplinary; Chemistry, Applied; Food Science & Technology SC Agriculture; Chemistry; Food Science & Technology GA DP0QI UT WOS:000378193900005 PM 27236926 ER PT J AU Zhang, DD Yang, YM Bekenstein, Y Yu, Y Gibson, NA Wong, AB Eaton, SW Kornienko, N Kong, Q Lai, ML Alivisatos, AP Leone, SR Yang, PD AF Zhang, Dandan Yang, Yiming Bekenstein, Yehonadav Yu, Yi Gibson, Natalie A. Wong, Andrew B. Eaton, Samuel W. Kornienko, Nikolay Kong, Qiao Lai, Minliang Alivisatos, A. Paul Leone, Stephen R. Yang, Peidong TI Synthesis of Composition Tunable and Highly Luminescent Cesium Lead Halide Nanowires through Anion-Exchange Reactions SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID PEROVSKITE NANOWIRES; IODIDE PEROVSKITE; CATION-EXCHANGE; NANOCRYSTALS; CSPBX3; ARRAYS; PHASE; BR; CL AB Here, we demonstrate the successful syn.= thesis of brightly emitting colloidal cesium lead halide (CsPbX3, X = Cl, Br, I) nanowires (NWs) with uniform diameters and tunable compositions. By using highly monodisperse CsPbBr3 NWs as templates, the NW composition can be independently controlled through anion-exchange reactions. CsPbX3 alloy NWs with a wide range of alloy compositions can be achieved with wellpreserved morphology and crystal structure. The NI/Vs are highly luminescent with photoluminescence quantum yields (PLQY) ranging from 20% to 80%. The bright photoluminescence can be tuned over nearly the entire visible spectrum. The high PLQYs together with charge transport measurements exemplify the efficient alloying of the anionic sublattice in a one-dimensional CsPbX3 system. The wires increased functionality in the form of fast photoresponse rates and the low defect density suggest CsPbX3 NWs as prospective materials for,optoelectronic applications. C1 [Zhang, Dandan; Yang, Yiming; Bekenstein, Yehonadav; Yu, Yi; Gibson, Natalie A.; Wong, Andrew B.; Eaton, Samuel W.; Kornienko, Nikolay; Kong, Qiao; Lai, Minliang; Alivisatos, A. Paul; Leone, Stephen R.; Yang, Peidong] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Alivisatos, A. Paul; Yang, Peidong] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Leone, Stephen R.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Zhang, Dandan; Yang, Yiming; Bekenstein, Yehonadav; Yu, Yi; Wong, Andrew B.; Alivisatos, A. Paul; Yang, Peidong] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Gibson, Natalie A.; Leone, Stephen R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Bekenstein, Yehonadav; Alivisatos, A. Paul; Yang, Peidong] Kavli Energy NanoSci Inst, Berkeley, CA 94720 USA. RP Yang, PD (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Yang, PD (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA.; Yang, PD (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.; Yang, PD (reprint author), Kavli Energy NanoSci Inst, Berkeley, CA 94720 USA. EM p_yang@berkeley.edu RI Alivisatos , Paul /N-8863-2015 OI Alivisatos , Paul /0000-0001-6895-9048 FU U.S. Department of Energy [DE-AC02-05CH11231]; office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231]; Suzhou Industrial Park; Camille and Henry Dreyfus Foundation [EP-14-151] FX This work was supported by the Director, Office of Science, Office of Basic Energy Sciences, Materials Science and Engineering Division, U.S. Department of Energy under contract no. DE-AC02-05CH11231 (P-Chem). Work at the Molecular Foundry was supported by the office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy under contract no. DE-AC02-05CH11231. D.Z. would like to thank the fellowship support from Suzhou Industrial Park. S.W.E. would like to thank the Camille and Henry Dreyfus Foundation for funding, award no. EP-14-151. NR 28 TC 26 Z9 26 U1 57 U2 152 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUN 15 PY 2016 VL 138 IS 23 BP 7236 EP 7239 DI 10.1021/jacs.6b03134 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA DP0QC UT WOS:000378193300008 PM 27213511 ER PT J AU Wu, QH Zhao, DL Schneider, AM Chen, W Yu, LP AF Wu, Qinghe Zhao, Donglin Schneider, Alexander M. Chen, Wei Yu, Luping TI Covalently Bound Clusters of Alpha-Substituted PDI-Rival Electron Acceptors to Fullerene for Organic Solar Cells SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID SMALL-MOLECULE ACCEPTOR; HIGH-EFFICIENCY; NONFULLERENE ACCEPTOR; 3D STRUCTURE; PHOTOVOLTAICS AB A cluster type of electron acceptor, TPB, bearing four alpha-perylenediimides (PDIs), was developed, in which the four PDIs form a cross-like molecular conformation while still partially conjugated with the BDT-Th core. The blend TPB:PTB7-Th films show favorable morphology and efficient charge dissociation. The inverted solar cells exhibited the highest PCE of 8.47% with the extraordinarily high Js, values (>18 mA/cm(2)), comparable with those of the corresponding PC7IBM/PTB7-Th-based solar cells. C1 [Wu, Qinghe; Zhao, Donglin; Schneider, Alexander M.; Yu, Luping] Univ Chicago, Dept Chem, 929 E 57th St, Chicago, IL 60637 USA. [Wu, Qinghe; Zhao, Donglin; Schneider, Alexander M.; Yu, Luping] Univ Chicago, James Franck Inst, 929 E 57th St, Chicago, IL 60637 USA. [Chen, Wei] Argonne Natl Lab, Div Mat Sci, 9700 Cass Ave, Lemont, IL 60439 USA. [Chen, Wei] Univ Chicago, Inst Mol Engn, 5747 South Ellis Ave, Chicago, IL 60637 USA. RP Yu, LP (reprint author), Univ Chicago, Dept Chem, 929 E 57th St, Chicago, IL 60637 USA.; Yu, LP (reprint author), Univ Chicago, James Franck Inst, 929 E 57th St, Chicago, IL 60637 USA. EM lupingyu@uchicago.edu RI Chen, Wei/G-6055-2011 OI Chen, Wei/0000-0001-8906-4278 FU U.S. National Science Foundation [NSF DMR-1263006]; NSF MRSEC program at the University of Chicago [DMR-0213745]; DOE via the ANSER Center, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001059]; NIST via CHIMAD program; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work was supported by U.S. National Science Foundation grant (NSF DMR-1263006) and NSF MRSEC program at the University of Chicago (DMR-0213745), DOE via the ANSER Center, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under award no. DE-SC0001059 and NIST via CHIMAD program. Use of the Advanced Photon Source (APS) at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under contract no. DE-AC02-06CH11357. NR 27 TC 39 Z9 39 U1 20 U2 47 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUN 15 PY 2016 VL 138 IS 23 BP 7248 EP 7251 DI 10.1021/jacs.6b03562 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA DP0QC UT WOS:000378193300011 PM 27219665 ER PT J AU Petrie, JR Jeen, H Barron, SC Meyer, TL Lee, HN AF Petrie, Jonathan R. Jeen, Hyoungjeen Barron, Sara C. Meyer, Tricia L. Lee, Ho Nyung TI Enhancing Perovskite Electrocatalysis through Strain Tuning of the Oxygen Deficiency SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID REDOX REACTIONS; EVOLUTION; SURFACE; OXIDES; STABILITY; CATALYSTS; DEFECTS; REACTIVITY; TIO2(110); DIFFUSION AB Oxygen vacancies in transition-metal oxides facilitate catalysis critical for energy storage and generation. However, promoting vacancies at the lower temperatures required for operation in devices such as metal air batteries and portable fuel cells has proven elusive. Here we used thin films of perovskite-based strontium cobaltite (SrCoOx) to show that epitaxial strain is a powerful tool for manipulating the Oxygen content under condition consistent with the oxygen evolution reaction, yielding increasingly oxygen-deficient states in an environment where the cobaltite would normally be fully oxidized: The additional oxygen vacancies created through tensile strain enhance the cobaltite's catalytic activity toward this important reaction by over an order of magnitude, equaling that of precious-metal catalysts, including IrO2. Our findings demonstrate that strain in. these oxides can dictate the oxygen stoichiometry independent of ambient conditions, allowing unprecedented control over oxygen vacancies essential in catalysis near room temperature. C1 [Petrie, Jonathan R.; Jeen, Hyoungjeen; Meyer, Tricia L.; Lee, Ho Nyung] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Barron, Sara C.] NIST, 100 Bur Dr, Gaithersburg, MD 20899 USA. RP Lee, HN (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. EM hnlee@ornl.gov FU Laboratory Directed Research and Development Program of Oak Ridge National Laboratory; U.S. DOE, Office of Science, Basic Energy Sciences, Materials Science and Engineering Division (synthesis and physical property characterization) FX This work was supported by the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy (DOE) (electrochemical characterization) and by the U.S. DOE, Office of Science, Basic Energy Sciences, Materials Science and Engineering Division (synthesis and physical property characterization). Reference electrode depositions were performed as a user project at the Center for Nanophase Materials Sciences, a DOE Office of Science User Facility. NR 35 TC 4 Z9 4 U1 40 U2 109 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUN 15 PY 2016 VL 138 IS 23 BP 7252 EP 7255 DI 10.1021/jacs.6b03520 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA DP0QC UT WOS:000378193300012 PM 27232374 ER PT J AU Bera, MK Antonio, MR AF Bera, Mrinal K. Antonio, Mark R. TI Crystallization of Keggin Heteropolyanions via a Two-Step Process in Aqueous Solutions SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID EFFECTIVE NUCLEUS; PROTEIN CRYSTALS; NUCLEATION; MECHANISM; GROWTH; ACID; SEPARATION; CLUSTERS; HYDROGEN; MODELS AB Although the analytical simplicity of the one-step classical theory of nucleation facilitates its use to understand crystallization processes, recent experiments and simulations have shown that many occur via multiple steps. According to the contemporary two-stage theory of nucleation, the onset of crystallization in a solution is preceded by large density, fluctuations in the mother liquor that results in the formation of dense liquid-like correlated structures of the constituent solute particles. Here we report the observation of dense liquid-like correlated structures of heteropolyadd salts of alpha-Keggin anions (heterepolyanions) in aqueous solutions as volume is decreased long before the onset of crystallization by in situ time-dependent small-angle X-ray scattering measurements. Experiments were performed on drying drops of solutions of heteropolyacids to, monitor their ordering before and during the onset of their crystallization. A continuous change in the density of the correlated structures is observed up to the onset of crystallization. Moreover, the correlated structures and the onset of crystallization are found to depend upon the charge of the heteropolyanions. The crystals formed within the drying drops of solutions during the crystallization process are found to be metastable polymorphic structures that are different from the stable crystal structures obtained after complete drying of the drops. Our results support,a two-step process and Ostwald's of stages for the crystallization of heteropolyanions in their aqueous solutions upon evaporation. C1 [Bera, Mrinal K.; Antonio, Mark R.] Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Bera, Mrinal K.] European Synchrotron Radiat Facil, DUBBLE CRG, CS40220, F-38043 Grenoble 9, France. RP Bera, MK; Antonio, MR (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA.; Bera, MK (reprint author), European Synchrotron Radiat Facil, DUBBLE CRG, CS40220, F-38043 Grenoble 9, France. EM mrinal.bera@esrf.fr; mantonio@anl.gov FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Biosciences and Geosciences [DE-AC02-06CH11357] FX We thank our Argonne colleague Dr. Soenke Seifert for assistance with small-angle X-ray scattering experiments and Dr. Benjamin Burton-Pye (Lehman College) for the synthesis of aluminotungstic acid. This work and the use of the Advanced Photon Source are supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Biosciences and Geosciences, under contract No DE-AC02-06CH11357. NR 40 TC 6 Z9 6 U1 11 U2 20 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUN 15 PY 2016 VL 138 IS 23 BP 7282 EP 7288 DI 10.1021/jacs.5b13375 PG 7 WC Chemistry, Multidisciplinary SC Chemistry GA DP0QC UT WOS:000378193300019 PM 27249015 ER PT J AU Sanders, SN Kumarasamy, E Pun, AB Appavoo, K Steigerwald, ML Campos, LM Sfeir, MY AF Sanders, Samuel N. Kumarasamy, Elango Pun, Andrew B. Appavoo, Kannatassen Steigerwald, Michael L. Campos, Luis M. Sfeir, Matthew Y. TI Exciton Correlations in Intramolecular Singlet Fission SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID TRIPLET-TRIPLET ANNIHILATION; SOLAR-ENERGY CONVERSION; PENTACENE DIMERS; DELAYED FLUORESCENCE; GAP LAW; STATES; EFFICIENCY; TETRACENE; DERIVATIVES; MOLECULES AB We have synthesized a series of asymmetric pentacene tetracene heterodimers with a variable-length conjugated bridge that undergo fast and efficient intramolecular singlet fission (iSF). These compounds have distinct singlet and triplet energies, which allow us to study the spatial dynamics of excitons during the iSF process, including the significant role of exciton correlations in promoting triplet pair generation and recombination. We demonstrate that the primary photo excitations in conjugated dialers are delocalized singlets that enable fast and efficient iSF. However, in these asymmetric dimers, the singlet becomes more localized on the lower energy unit as the length of the bridge is increased, slowing down iSF relative to analogous symmetric dimers. We resolve the recombination kinetics of the inequivalent triplets produced via iSF, and find that they primarily decay via concerted processes. By identifying different decay "channels, including delayed fluorescence via triplet triplet annihilation, we can separate transient species corresponding to both correlated triplet pairs and uncorrelated triplets. Recombination of the triplet pair proceeds rapidly despite our experimental and theoretical demonstration that individual triplets are highly localized and unable to be transported across the conjugated linker. In this class of compounds, the rate of formation and yield of uncorrelated "triplets increases with bridge length. Overall, these "constrained, asymmetric systems provide a unique platform to isolate and study transient species essential for singlet fission, which are otherwise difficult to observe in symmetric dimers or condensed phases. C1 [Sanders, Samuel N.; Kumarasamy, Elango; Pun, Andrew B.; Steigerwald, Michael L.; Campos, Luis M.] Columbia Univ, Dept Chem, New York, NY 10027 USA. [Appavoo, Kannatassen; Sfeir, Matthew Y.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Campos, LM (reprint author), Columbia Univ, Dept Chem, New York, NY 10027 USA.; Sfeir, MY (reprint author), Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. EM lcampos@columbia.edu; msfeir@bnl.gov OI Pun, Andrew/0000-0002-3052-912X; Kumarasamy, Elango/0000-0002-7995-6894 FU Office of Naval Research Young Investigator Program [N00014-15-1-2532]; ACS Petroleum Research Fund; 3M Non-Tenured Faculty Award; Arthur C. Cope Scholar Award; Cottrell Scholar Award; NSF [DGE 11-44155]; U.S. DOE Office of Science Facility, at Brookhaven National Laboratory [DE-SC0012704] FX We thank Timothy John Harvey Hele, Eric Fuemmeler, and Nandini Ananth for useful discussions concerning the electronic structure of covalent dimers. L.M.C. acknowledges support from the Office of Naval Research Young Investigator Program (Award N00014-15-1-2532), ACS Petroleum Research Fund, 3M Non-Tenured Faculty Award, Arthur C. Cope Scholar Award, and Cottrell Scholar Award. S.N.S. and A.B.P. thank the NSF for GRFP (DGE 11-44155). This research used resources of the Center for Functional Nanomaterials, which is a U.S. DOE Office of Science Facility, at Brookhaven National Laboratory under Contract No. DE-SC0012704. We are grateful to the Nuckolls lab for use of their UV-vis spectrophotometer. NR 56 TC 8 Z9 8 U1 29 U2 64 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUN 15 PY 2016 VL 138 IS 23 BP 7289 EP 7297 DI 10.1021/jacs.6b00657 PG 9 WC Chemistry, Multidisciplinary SC Chemistry GA DP0QC UT WOS:000378193300020 PM 27183040 ER PT J AU Han, TH Isaacs, ED Schlueter, JA Singleton, J AF Han, Tian-Heng Isaacs, Eric D. Schlueter, John A. Singleton, John TI Anisotropy: Spin order and magnetization of single-crystalline Cu-4(OH)(6)FBr barlowite SO PHYSICAL REVIEW B LA English DT Article ID LATTICE; LIQUID; ANTIFERROMAGNET; STATE AB Despite decades-long fascination, the difficulty of maintaining high lattice symmetry in frustrated nonbipartite S = 1/2 materials that can also be made into high-quality single crystals has been a persistent challenge. Here we report magnetization studies of a single-crystal sample of barlowite, Cu-4(OH)(6)FBr, which has a geometrically perfect kagome motif. At T <= 4.2 K and 35 <= mu H-0 <= 65 T, the interlayer spins are fully polarized, and the kagome-intrinsic magnetization is consistent with a Heisenberg model having J/k(B) = -180 K. Several field-driven anomalies are observed, having varied scalings with temperature. At an applied field, kagome disorder caused by the interlayer spins is smaller than that in herbertsmithite. At T <= 15 K, the bulk magnetic moment comes from the interlayer spins. An almost coplanar spin order suggests that the magnitude of in-plane Dzyaloshinskii-Moriya interaction is smaller than 0.006(6) J. On the other hand, the possibility of a spin-liquid state in the kagome lattice coexisting with ordered interlayer spins is left open. C1 [Han, Tian-Heng; Isaacs, Eric D.] Univ Chicago, James Franck Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Han, Tian-Heng; Isaacs, Eric D.] Univ Chicago, Dept Phys, Chicago, IL 60637 USA. [Han, Tian-Heng; Schlueter, John A.] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. [Schlueter, John A.] Natl Sci Fdn, Div Mat Res, 4201 Wilson Blvd, Arlington, VA 22230 USA. [Singleton, John] Los Alamos Natl Lab, Natl High Magnet Field Lab, POB 1663, Los Alamos, NM 87545 USA. RP Han, TH (reprint author), Univ Chicago, James Franck Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA.; Han, TH (reprint author), Univ Chicago, Dept Phys, Chicago, IL 60637 USA. EM tianheng@alum.mit.edu FU Department of Physics, University of Chicago; Department of Energy (DOE) [DE-FG02-99ER45789, DE-AC02-06CH11357]; NSF Independent Research/Development program; NSF [DMR-1157490]; State of Florida; DOE; DOE Basic Energy Science Field Work Proposal "Science in 100 T" FX We thank P. Lee, D. Huse, Y. Takano, and T. Rosenbaum for careful reading with useful comments. T.-H. H. acknowledges the support of the Grainger Fellowship provided by the Department of Physics, University of Chicago and the support from the Department of Energy (DOE) (Grants No. DE-FG02-99ER45789 and No. DE-AC02-06CH11357). J.A.S. acknowledges support from the NSF Independent Research/Development program. A portion of this work was performed at the National High Magnetic Field Laboratory, which is supported by NSF Cooperative Agreement No. DMR-1157490, the State of Florida, the DOE, and through the DOE Basic Energy Science Field Work Proposal "Science in 100 T". NR 35 TC 1 Z9 1 U1 17 U2 22 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUN 15 PY 2016 VL 93 IS 21 AR 214416 DI 10.1103/PhysRevB.93.214416 PG 6 WC Physics, Condensed Matter SC Physics GA DO5BB UT WOS:000377797500003 ER PT J AU Lopez-Bezanilla, A Littlewood, PB AF Lopez-Bezanilla, Alejandro Littlewood, Peter B. TI Electronic properties of 8-Pmmn borophene SO PHYSICAL REVIEW B LA English DT Article ID WANNIER FUNCTIONS AB First-principles calculations on monolayer 8-Pmmn borophene are reported to reveal unprecedented electronic properties in a two-dimensional material. Based on a Born effective charge analysis, 8-Pmmn borophene is the first single-element-based monolayered material exhibiting two sublattices with substantial ionic features. The observed Dirac cones are actually formed by the p(z) orbitals of one of the inequivalent sublattices composed of uniquely four atoms, yielding an underlying hexagonal network topologically equivalent to distorted graphene. A significant physical outcome of this effect includes the possibility of converting metallic 8-Pmmn borophene into an indirect band gap semiconductor by means of external shear stress. The stability of the strained structures are supported by a phonon frequency analysis. The Dirac cones are sensitive to the formation of vacancies only in the inequivalent sublattice electronically active at the Fermi level. C1 [Lopez-Bezanilla, Alejandro; Littlewood, Peter B.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Littlewood, Peter B.] Univ Chicago, James Franck Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. RP Lopez-Bezanilla, A (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. EM alejandrolb@gmail.com RI Lopez-Bezanilla, Alejandro/B-9125-2015 OI Lopez-Bezanilla, Alejandro/0000-0002-4142-2360 FU DOE BES Glue [FWP 70081]; DOE-BES [DE-AC02-06CH11357] FX We acknowledge DOE BES Glue funding through Grant No. FWP 70081. We acknowledge the computing resources provided on Blues high-performance computing cluster operated by the Laboratory Computing Resource Center at Argonne National Laboratory. Work at Argonne is supported by DOE-BES under Contract No. DE-AC02-06CH11357. NR 16 TC 3 Z9 3 U1 30 U2 70 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUN 15 PY 2016 VL 93 IS 24 AR 241405 DI 10.1103/PhysRevB.93.241405 PG 5 WC Physics, Condensed Matter SC Physics GA DO5DB UT WOS:000377802700006 ER PT J AU Doring, M Revier, J Ronchen, D Workman, RL AF Doring, M. Revier, J. Ronchen, D. Workman, R. L. TI Correlations of pi N partial waves for multireaction analyses SO PHYSICAL REVIEW C LA English DT Article ID CHIRAL PERTURBATION-THEORY; MESON-NUCLEON SCATTERING; ELASTIC-SCATTERING; ETA-PHOTOPRODUCTION; BARYON RESONANCES; FIELD-THEORY; UNITARY; DYNAMICS; MODEL; AMPLITUDES AB In the search for missing baryonic resonances, many analyses include data from a variety of pion- and photon-induced reactions. For elastic pi N scattering, however, usually the partial waves of the SAID (Scattering Analysis Interactive Database) or other groups are fitted, instead of data. We provide the partial-wave covariance matrices needed to perform correlated chi(2) fits, in which the obtained chi(2) equals the actual chi(2) up to nonlinear and normalization corrections. For any analysis relying on partial waves extracted from elastic pion scattering, this is a prerequisite to assess the significance of resonance signals and to assign any uncertainty on results. The influence of systematic errors is also considered. C1 [Doring, M.] George Washington Univ, Inst Nucl Studies, Astron Phys & Stat Inst Sci, Dept Phys, 725 21st St NW, Washington, DC 20052 USA. [Doring, M.] Thomas Jefferson Natl Accelerator Facil, 12000 Jefferson Ave, Newport News, VA 23606 USA. [Revier, J.] George Washington Univ, Dept Phys, 725 21st St NW, Washington, DC 20052 USA. [Ronchen, D.] Univ Bonn, Helmholtz Inst Strahlen & Kernphys Theorie, D-53115 Bonn, Germany. [Ronchen, D.] Univ Bonn, Bethe Ctr Theoret Phys, D-53115 Bonn, Germany. [Workman, R. L.] George Washington Univ, Inst Nucl Studies, 20101 Acad Way, Ashburn, VA 20147 USA. [Workman, R. L.] George Washington Univ, Dept Phys, 20101 Acad Way, Ashburn, VA 20147 USA. RP Doring, M (reprint author), George Washington Univ, Inst Nucl Studies, Astron Phys & Stat Inst Sci, Dept Phys, 725 21st St NW, Washington, DC 20052 USA.; Doring, M (reprint author), Thomas Jefferson Natl Accelerator Facil, 12000 Jefferson Ave, Newport News, VA 23606 USA. EM doring@gwu.edu; rworkman@gwu.edu FU U.S. Department of Energy [DE-SC0014133]; National Science Foundation [1452055, 1415459]; GWU (startup grant); DFG; NSFC through the Sino-German CRC [110] FX This work was supported in part by the U.S. Department of Energy Grant No. DE-SC0014133, by the National Science Foundation (CAREER Grant No. 1452055, PIF Grant No. 1415459), by GWU (startup grant), and by the DFG and NSFC through the Sino-German CRC 110. The authors gratefully acknowledge the computing time granted on the supercomputer JURECA at Julich Supercomputing Centre (JSC, Forschungszentrum Julich) and thank Cesar Fernandez Ramirez for useful discussions. NR 68 TC 2 Z9 2 U1 1 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD JUN 15 PY 2016 VL 93 IS 6 AR 065205 DI 10.1103/PhysRevC.93.065205 PG 7 WC Physics, Nuclear SC Physics GA DO5DL UT WOS:000377803700001 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Asilar, E Bergauer, T Brandstetter, J Brondolin, E Dragicevic, M Ero, J Flechl, M Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Knunz, V Konig, A Krammer, M Kratschmer, I Liko, D Matsushita, T Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schieck, J Schofbeck, R Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Lauwers, J Luyckx, S Ochesanu, S Rougny, R Van de Klundert, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Abu Zeid, S Blekman, F D'Hondt, J Daci, N De Bruyn, I Deroover, K Heracleous, N Keaveney, J Lowette, S Moreels, L Olbrechts, A Python, Q Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Van Parijs, I Barria, P Caillol, C Clerbaux, B De Lentdecker, G Delannoy, H Dobur, D Fasanella, G Favart, L Gay, APR Grebenyuk, A Lenzi, T Leonard, A Maerschalk, T Mohammadi, A Pernie, L Randle-conde, A Reis, T Seva, T Vander Velde, C Vanlaer, P Wang, J Yonamine, R Zenoni, F Zhang, F Beernaert, K Benucci, L Cimmino, A Crucy, S Fagot, A Garcia, G Gul, M Mccartin, J Rios, AAO Poyraz, D Ryckbosch, D Salva, S Sigamani, M Strobbe, N Tytgat, M Van Driessche, W Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bondu, O Bruno, G Castello, R Caudron, A Ceard, L Da Silveira, GG Delaere, C Favart, D Forthomme, L Giammanco, A Hollar, J Jafari, A Jez, P Komm, M Lemaitre, V Mertens, A Nuttens, C Perrini, L Pin, A Piotrzkowski, K Popov, A Quertenmont, L Selvaggi, M Marono, MV Beliy, N Caebergs, T Hammad, GH Alda, WL Alves, GA Brito, L Martins, MC Martins, TD Hensel, C Herrera, CM Moraes, A Pol, ME Teles, PR Das Chagas, EBB Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD De Souza, SF Guativa, LMH Malbouisson, H Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santoro, A Sznajder, A Manganote, EJT Pereira, AV Ahuja, S Bernardes, CA Santos, AD Dogra, S Tomei, TRFP Gregores, EM Mercadante, PG Moon, CS Novaes, SF Padula, SA Abad, DR Vargas, JCR Aleksandrov, A Genchev, V Hadjiiska, R Iaydjiev, P Marinov, A Piperov, S Rodozov, M Stoykova, S Sultanov, G Vutova, M Dimitrov, A Glushkov, I Litov, L Pavlov, B Petkov, P Ahmad, M Bian, JG Chen, GM Chen, HS Chen, M Cheng, T Du, R Jiang, CH Plestina, R Romeo, F Shaheen, SM Tao, J Wang, C Wang, Z Zhang, H Asawatangtrakuldee, C Ban, Y Li, Q Liu, S Mao, Y Qian, SJ Wang, D Xu, Z Zou, W Avila, C Cabrera, A Sierra, LFC Florez, C Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Polic, D Puljak, I Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Sudic, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Rykaczewski, H Bodlak, M Finger, M Finger, M Aly, R Aly, S Assran, Y Elgammal, S Kamel, AE Lotfy, A Mahmoud, MA Radi, A Sayed, A Calpas, B Kadastik, M Murumaa, M Raidal, M Tiko, A Veelken, C Eerola, P Pekkanen, J Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E Wendland, L Talvitie, J Tuuva, T Besancon, M Couderc, F Dejardin, M Denegri, D Fabbro, B Faure, JL Favaro, C Ferri, F Ganjour, S Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Machet, M Malcles, J Rander, J Rosowsky, A Titov, M Zghiche, A Baffioni, S Beaudette, F Busson, P Cadamuro, L Chapon, E Charlot, C Dahms, T Davignon, O Filipovic, N Florent, A de Cassagnac, RG Lisniak, S Mastrolorenzo, L Mine, P Naranjo, IN Nguyen, M Ochando, C Ortona, G Paganini, P Regnard, S Salerno, R Sauvan, JB Sirois, Y Strebler, T Yilmaz, Y Zabi, A Agram, JL Andrea, J Aubin, A Bloch, D Brom, JM Buttignol, M Chabert, EC Chanon, N Collard, C Conte, E Coubez, X Fontaine, JC Gele, D Goerlach, U Goetzmann, C Le Bihan, AC Merlin, JA Skovpen, K Van Hove, P Gadrat, S Beauceron, S Bernet, C Boudoul, G Bouvier, E Brochet, S Montoya, CAC Chasserat, J Chierici, R Contardo, D Courbon, B Depasse, P El Mamouni, H Fan, J Fay, J Gascon, S Gouzevitch, M Ille, B Laktineh, IB Lethuillier, M Mirabito, L Pequegnot, AL Perries, S Alvarez, JDR Sabes, D Sgandurra, L Sordini, V Vander Donckt, M Verdier, P Viret, S Xiao, H Toriashvili, T Tsamalaidze, Z Autermann, C Beranek, S Edelhoff, M Feld, L Heister, A Kiesel, MK Klein, K Lipinski, M Ostapchuk, A Preuten, M Raupach, F Sammet, J Schael, S Schulte, JF Verlage, T Weber, H Wittmer, B Zhukov, V Ata, M Brodski, M Dietz-Laursonn, E Duchardt, D Endres, M Erdmann, M Erdweg, S Esch, T Fischer, R Guth, A Hebbeker, T Heidemann, C Hoepfner, K Klingebiel, D Knutzen, S Kreuzer, P Merschmeyer, M Meyer, A Millet, P Olschewski, M Padeken, K Papacz, P Pook, T Radziej, M Reithler, H Rieger, M Scheuch, F Sonnenschein, L Teyssier, D Thuer, S Cherepanov, V Erdogan, Y Flugge, G Geenen, H Geisler, M Ahmad, WH Hoehle, F Kargoll, B Kress, T Kuessel, Y Kunsken, A Lingemann, J Nehrkorn, A Nowack, A Nugent, IM Pistone, C Pooth, O Stahl, A Martin, MA Asin, I Bartosik, N Behnke, O Behrens, U Bell, AJ Borras, K Burgmeier, A Cakir, A Calligaris, L Campbell, A Choudhury, S Costanza, F Pardos, CD Dolinska, G Dooling, S Dorland, T Eckerlin, G Eckstein, D Eichhorn, T Flucke, G Gallo, E Garcia, JG Geiser, A Gizhko, A Gunnellini, P Hauk, J Hempel, M Jung, H Kalogeropoulos, A Karacheban, O Kasemann, M Katsas, P Kieseler, J Kleinwort, C Korol, I Lange, W Leonard, J Lipka, K Lobanov, A Lohmann, W Mankel, R Marfin, I Melzer-Pellmann, IA Meyer, AB Mittag, G Mnich, J Mussgiller, A Naumann-Emme, S Nayak, A Ntomari, E Perrey, H Pitzl, D Placakyte, R Raspereza, A Cipriano, PMR Roland, B Sahin, MO Salfeld-Nebgen, J Saxena, P Schoerner-Sadenius, T Schroder, M Seitz, C Spannagel, S Trippkewitz, KD Wissing, C Blobel, V Vignali, MC Draeger, AR Erfle, J Garutti, E Goebel, K Gonzalez, D Gorner, M Haller, J 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Ferencek, D. Gershtein, Y. Gray, R. Halkiadakis, E. Hidas, D. Hughes, E. Kaplan, S. Elayavalli, R. Kunnawalkam Lath, A. Panwalkar, S. Park, M. Salur, S. Schnetzer, S. Sheffield, D. Somalwar, S. Stone, R. Thomas, S. Thomassen, P. Walker, M. Foerster, M. Riley, G. Rose, K. Spanier, S. York, A. Bouhali, O. Hernandez, A. Castaneda Dalchenko, M. De Mattia, M. Delgado, A. Dildick, S. Eusebi, R. Flanagan, W. Gilmore, J. Kamon, T. Krutelyov, V. Montalvo, R. Mueller, R. Osipenkov, I. Pakhotin, Y. Patel, R. Perloff, A. Roe, J. Rose, A. Safonov, A. Tatarinov, A. Ulmer, K. A. Akchurin, N. Cowden, C. Damgov, J. Dragoiu, C. Dudero, P. R. Faulkner, J. Kunori, S. Lamichhane, K. Lee, S. W. Libeiro, T. Undleeb, S. Volobouev, I. Appelt, E. Delannoy, A. G. Greene, S. Gurrola, A. Janjam, R. Johns, W. Maguire, C. Mao, Y. Melo, A. Sheldon, P. Snook, B. Tuo, S. Velkovska, J. Xu, Q. Arenton, M. W. Boutle, S. Cox, B. Francis, B. Goodell, J. Hirosky, R. Ledovskoy, A. Li, H. Lin, C. Neu, C. Wolfe, E. Wood, J. Xia, F. Clarke, C. Harr, R. Karchin, P. E. Don, C. Kottachchi Kankanamge Lamichhane, P. Sturdy, J. Belknap, D. A. Carlsmith, D. Cepeda, M. Christian, A. Dasu, S. Dodd, L. Duric, S. Friis, E. Gomber, B. Hall-Wilton, R. Herndon, M. Herve, A. Klabbers, P. Lanaro, A. Levine, A. Long, K. Loveless, R. Mohapatra, A. Ojalvo, I. Perry, T. Pierro, G. A. Polese, G. Ross, I. Ruggles, T. Sarangi, T. Savin, A. Sharma, A. Smith, N. Smith, W. H. Taylor, D. Woods, N. CA CMS Collaboration TI Search for pair-produced vectorlike B quarks in proton-proton collisions at root s=8 TeV SO PHYSICAL REVIEW D LA English DT Article ID TOP-PAIR; HIGGS; BOSON; RESUMMATION; MODEL; LHC AB A search for the production of a heavy B quark, having electric charge -1/3 and vector couplings to W, Z, and H bosons, is carried out using proton-proton collision data recorded at the CERN LHC by the CMS experiment, corresponding to an integrated luminosity of 19.7 fb(-1). The B quark is assumed to be pair produced and to decay in one of three ways: to tW, bZ, or bH. The search is carried out in final states with one, two, and more than two charged leptons, as well as in fully hadronic final states. Each of the channels in the exclusive final-state topologies is designed to be sensitive to specific combinations of the B quark-antiquark pair decays. The observed event yields are found to be consistent with the standard model expectations in all the final states studied. A statistical combination of these results is performed, and upper limits are set on the cross section of the strongly produced B quark-antiquark pairs as a function of the B quark mass. Lower limits on the B quark mass between 740 and 900 GeVare set at a 95% confidence level, depending on the values of the branching fractions of the B quark to tW, bZ, and bH. Overall, these limits are the most stringent to date. C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Asilar, E.; Bergauer, T.; Brandstetter, J.; Brondolin, E.; Dragicevic, M.; Eroe, J.; Flechl, M.; Friedl, M.; Fruehwirth, R.; Ghete, V. M.; Hartl, C.; Hoermann, N.; Hrubec, J.; Jeitler, M.; Knuenz, V.; Koenig, A.; Krammer, M.; Kratschmer, I.; Liko, D.; Matsushita, T.; Mikulec, I.; Rabady, D.; Rahbaran, B.; Rohringer, H.; Schieck, J.; Schoefbeck, R.; Strauss, J.; Treberer-Treberspurg, W.; Waltenberger, W.; Wulz, C-E.] Inst Hochenergiephys OeAW, Vienna, Austria. [Mossolov, V.; Shumeiko, N.; Gonzalez, J. Suarez] Natl Ctr Particle & High Energy Phys, Minsk, Byelarus. [Alderweireldt, S.; Cornelis, T.; De Wolf, E. A.; Janssen, X.; Knutsson, A.; Lauwers, J.; Luyckx, S.; Ochesanu, S.; Rougny, R.; Van de Klundert, M.; Van Haevermaet, H.; Van Mechelen, P.; Van Remortel, N.; Van Spilbeeck, A.] Univ Antwerp, B-2020 Antwerp, Belgium. [Abu Zeid, S.; Blekman, F.; D'Hondt, J.; Daci, N.; De Bruyn, I.; Deroover, K.; Heracleous, N.; Keaveney, J.; Lowette, S.; Moreels, L.; Olbrechts, A.; Python, Q.; Strom, D.; Tavernier, S.; Van Doninck, W.; Van Mulders, P.; Van Onsem, G. P.; Van Parijs, I.] Vrije Univ Brussel, Brussels, Belgium. [Barria, P.; Caillol, C.; Clerbaux, B.; De Lentdecker, G.; Delannoy, H.; Dobur, D.; Fasanella, G.; Favart, L.; Gay, A. P. R.; Grebenyuk, A.; Lenzi, T.; Leonard, A.; Maerschalk, T.; Mohammadi, A.; Pernie, L.; Randle-conde, A.; Reis, T.; Seva, T.; Vander Velde, C.; Vanlaer, P.; Wang, J.; Yonamine, R.; Zenoni, F.; Zhang, F.] Univ Libre Bruxelles, Brussels, Belgium. [Beernaert, K.; Benucci, L.; Cimmino, A.; Crucy, S.; Fagot, A.; Garcia, G.; Gul, M.; Mccartin, J.; Rios, A. A. Ocampo; Poyraz, D.; Ryckbosch, D.; Salva, S.; Sigamani, M.; Strobbe, N.; Tytgat, M.; Van Driessche, W.; Yazgan, E.; Zaganidis, N.] Univ Ghent, B-9000 Ghent, Belgium. [Basegmez, S.; Beluffi, C.; Bondu, O.; Bruno, G.; Castello, R.; Caudron, A.; Ceard, L.; Da Silveira, G. G.; Delaere, C.; Favart, D.; Forthomme, L.; Giammanco, A.; Hollar, J.; Jafari, A.; Jez, P.; Komm, M.; Lemaitre, V.; Mertens, A.; Nuttens, C.; Perrini, L.; Pin, A.; Piotrzkowski, K.; Popov, A.; Quertenmont, L.; Selvaggi, M.; Marono, M. Vidal] Catholic Univ Louvain, Louvain La Neuve, Belgium. [Beliy, N.; Caebergs, T.; Hammad, G. H.] Univ Mons, B-7000 Mons, Belgium. [Alda Junior, W. L.; Alves, G. A.; Brito, L.; Correa Martins Junior, M.; Dos Reis Martins, T.; Hensel, C.; Mora Herrera, C.; Moraes, A.; Pol, M. E.; Rebello Teles, P.] Ctr Brasileiro Pesquisas Fis, Rio De Janeiro, Brazil. [Belchior Batista Das Chagas, E.; Carvalho, W.; Chinellato, J.; Custodio, A.; Da Costa, E. M.; De Jesus Damiao, D.; De Oliveira Martins, C.; Fonseca De Souza, S.; Huertas Guativa, L. M.; Malbouisson, H.; Matos Figueiredo, D.; Mundim, L.; Nogima, H.; Prado Da Silva, W. L.; Santoro, A.; Sznajder, A.; Tonelli Manganote, E. J.; Vilela Pereira, A.] Univ Estado Rio de Janeiro, BR-20550011 Rio De Janeiro, Brazil. [Ahuja, S.; Dogra, S.; Fernandez Perez Tomei, T. R.; Moon, C. S.; Novaes, S. F.; Padula, Sandra A.; Romero Abad, D.; Ruiz Vargas, J. C.] Univ Estadual Paulista, Sao Paulo, Brazil. [Bernardes, C. A.; De Souza Santos, A.; Gregores, E. M.; Mercadante, P. G.] Univ Fed ABC, Sao Paulo, Brazil. [Aleksandrov, A.; Genchev, V.; Hadjiiska, R.; Iaydjiev, P.; Marinov, A.; Piperov, S.; Rodozov, M.; Stoykova, S.; Sultanov, G.; Vutova, M.] Bulgarian Acad Sci, Inst Nucl Res & Nucl Energy, Sofia, Bulgaria. [Dimitrov, A.; Glushkov, I.; Litov, L.; Pavlov, B.; Petkov, P.] Univ Sofia, BU-1126 Sofia, Bulgaria. [Ahmad, M.; Bian, J. G.; Chen, G. M.; Chen, H. S.; Chen, M.; Cheng, T.; Du, R.; Jiang, C. H.; Plestina, R.; Romeo, F.; Shaheen, S. M.; Tao, J.; Wang, C.; Wang, Z.; Zhang, H.] Inst High Energy Phys, Beijing 100039, Peoples R China. [Zhang, F.; Asawatangtrakuldee, C.; Ban, Y.; Li, Q.; Liu, S.; Mao, Y.; Qian, S. J.; Wang, D.; Xu, Z.; Zou, W.] Peking Univ, State Key Lab Nucl Phys & Technol, Beijing 100871, Peoples R China. [Avila, C.; Cabrera, A.; Chaparro Sierra, L. F.; Florez, C.; Gomez, J. P.; Gomez Moreno, B.; Sanabria, J. C.] Univ Los Andes, Bogota, Colombia. [Godinovic, N.; Lelas, D.; Polic, D.; Puljak, I.] Univ Split, Fac Elect Engn Mech Engn & Naval Architecture, Split, Croatia. [Antunovic, Z.; Kovac, M.] Univ Split, Fac Sci, Split, Croatia. [Brigljevic, V.; Kadija, K.; Luetic, J.; Sudic, L.] Rudjer Boskovic Inst, Zagreb, Croatia. [Attikis, A.; Mavromanolakis, G.; Mousa, J.; Nicolaou, C.; Ptochos, F.; Razis, P. A.; Rykaczewski, H.] Univ Cyprus, CY-1678 Nicosia, Cyprus. [Bodlak, M.; Finger, M.] Charles Univ Prague, Prague, Czech Republic. [Aly, R.; Aly, S.; Assran, Y.; Elgammal, S.; Kamel, A. Ellithi; Lotfy, A.; Mahmoud, M. A.; Radi, A.; Sayed, A.] Egyptian Network High Energy Phys, Acad Sci Res & Technol Arab Republ Egypt, Cairo, Egypt. [Giammanco, A.; Calpas, B.; Kadastik, M.; Murumaa, M.; Raidal, M.; Tiko, A.; Veelken, C.] NICPB, Tallinn, Estonia. [Eerola, P.; Pekkanen, J.; Voutilainen, M.] Univ Helsinki, Dept Phys, Helsinki, Finland. [Karimaki, V.; Kinnunen, R.; Lampen, T.; Lassila-Perini, K.; Lehti, S.; Linden, T.; Luukka, P.; Maenpaa, T.; Peltola, T.; Tuominen, E.; Tuominiemi, J.; Tuovinen, E.; Wendland, L.] Helsinki Inst Phys, Helsinki, Finland. [Talvitie, J.; Tuuva, T.] Lappeenranta Univ Technol, Lappeenranta, Finland. [Besancon, M.; Couderc, F.; Dejardin, M.; Denegri, D.; Fabbro, B.; Faure, J. L.; Favaro, C.; Ferri, F.; Ganjour, S.; Givernaud, A.; Gras, P.; de Monchenault, G. Hamel; Jarry, P.; Locci, E.; Machet, M.; Malcles, J.; Rander, J.; Rosowsky, A.; Titov, M.; Zghiche, A.] CEA Saclay, DSM IRFU, F-91191 Gif Sur Yvette, France. [Plestina, R.; Baffioni, S.; Beaudette, F.; Busson, P.; Cadamuro, L.; Chapon, E.; Charlot, C.; Dahms, T.; Davignon, O.; Filipovic, N.; Florent, A.; de Cassagnac, R. Granier; Lisniak, S.; Mastrolorenzo, L.; Mine, P.; Naranjo, I. N.; Nguyen, M.; Ochando, C.; Ortona, G.; Paganini, P.; Regnard, S.; Salerno, R.; Sauvan, J. B.; Sirois, Y.; Strebler, T.; Yilmaz, Y.; Zabi, A.] Ecole Polytech, CNRS, IN2P3, Lab Leprince Ringuet, F-91128 Palaiseau, France. [Beluffi, C.; Agram, J-L.; Andrea, J.; Aubin, A.; Bloch, D.; Brom, J-M.; Buttignol, M.; Chabert, E. C.; Chanon, N.; Collard, C.; Conte, E.; Coubez, X.; Fontaine, J-C.; Gele, D.; Goerlach, U.; Goetzmann, C.; Le Bihan, A-C.; Merlin, J. A.; Skovpen, K.; Van Hove, P.] Univ Haute Alsace Mulhouse, Univ Strasbourg, Inst Pluridisciplinaire Hubert Curien, CNRS,IN2P3, Strasbourg, France. [Gadrat, S.] Inst Natl Phys Nucl & Phys Particules, CNRS, IN2P3, Ctr Calcul, Villeurbanne, France. [Beauceron, S.; Bernet, C.; Boudoul, G.; Bouvier, E.; Brochet, S.; Montoya, C. A. Carrillo; Chasserat, J.; Chierici, R.; Contardo, D.; Courbon, B.; Depasse, P.; El Mamouni, H.; Fan, J.; Fay, J.; Gascon, S.; Gouzevitch, M.; Ille, B.; Laktineh, I. B.; Lethuillier, M.; Mirabito, L.; Pequegnot, A. L.; Perries, S.; Alvarez, J. D. Ruiz; Sabes, D.; Sgandurra, L.; Sordini, V.; Vander Donckt, M.; Verdier, P.; Viret, S.] Univ Lyon 1, CNRS, IN2P3, Inst Phys Nucl Lyon, F-69622 Villeurbanne, France. [Toriashvili, T.] Georgian Tech Univ, Tbilisi, Rep of Georgia. [Toriashvili, T.; Tsamalaidze, Z.] Tbilisi State Univ, GE-380086 Tbilisi, Rep of Georgia. [Autermann, C.; Beranek, S.; Edelhoff, M.; Feld, L.; Heister, A.; Kiesel, M. K.; Klein, K.; Lipinski, M.; Ostapchuk, A.; Preuten, M.; Raupach, F.; Sammet, J.; Schael, S.; Schulte, J. F.; Verlage, T.; Weber, H.; Wittmer, B.; Zhukov, V.] Rhein Westfal TH Aachen, Inst Phys 1, Aachen, Germany. [Ata, M.; Brodski, M.; Dietz-Laursonn, E.; Duchardt, D.; Endres, M.; Erdmann, M.; Erdweg, S.; Esch, T.; Fischer, R.; Gueth, A.; Hebbeker, T.; Heidemann, C.; Hoepfner, K.; Klingebiel, D.; Knutzen, S.; Kreuzer, P.; Merschmeyer, M.; Meyer, A.; Millet, P.; Olschewski, M.; Padeken, K.; Papacz, P.; Pook, T.; Radziej, M.; Reithler, H.; Rieger, M.; Scheuch, F.; Sonnenschein, L.; Teyssier, D.; Thueer, S.; Yi, K.] Rhein Westfal TH Aachen, Phys Inst A 3, Aachen, Germany. [Cherepanov, V.; Erdogan, Y.; Fluegge, G.; Geenen, H.; Geisler, M.; Ahmad, W. Haj; Hoehle, F.; Kargoll, B.; Kress, T.; Kuessel, Y.; Kuensken, A.; Lingemann, J.; Nehrkorn, A.; Nowack, A.; Nugent, I. M.; Pistone, C.; Pooth, O.; Stahl, A.] Rhein Westfal TH Aachen, Phys Inst A B, Aachen, Germany. [Martin, M. Aldaya; Asin, I.; Bartosik, N.; Behnke, O.; Behrens, U.; Bell, A. J.; Borras, K.; Burgmeier, A.; Cakir, A.; Calligaris, L.; Campbell, A.; Choudhury, S.; Costanza, F.; Pardos, C. Diez; Dolinska, G.; Dooling, S.; Dorland, T.; Eckerlin, G.; Eckstein, D.; Eichhorn, T.; Flucke, G.; Garcia, J. Garay; Geiser, A.; Gizhko, A.; Gunnellini, P.; Hauk, J.; Hempel, M.; Jung, H.; Kalogeropoulos, A.; Karacheban, O.; Kasemann, M.; Katsas, P.; Kieseler, J.; Kleinwort, C.; Korol, I.; Lange, W.; Leonard, J.; Lipka, K.; Lobanov, A.; Lohmann, W.; Mankel, R.; Marfin, I.; Melzer-Pellmann, I-A; Meyer, A. B.; Mittag, G.; Mnich, J.; Mussgiller, A.; Naumann-Emme, S.; Nayak, A.; Ntomari, E.; Perrey, H.; Pitzl, D.; Placakyte, R.; Raspereza, A.; Cipriano, P. M. Ribeiro; Roland, B.; Sahin, M. Oe; Salfeld-Nebgen, J.; Saxena, P.; Schoerner-Sadenius, T.; Schroeder, M.; Seitz, C.; Spannagel, S.; Trippkewitz, K. D.; Wissing, C.; Yi, K.] DESY, Hamburg, Germany. [Vignali, M. Centis; Draeger, A. R.; Erfle, J.; Garutti, E.; Goebel, K.; Gonzalez, D.; Goerner, M.; Haller, J.; Hoffmann, M.; Hoeing, R. S.; Junkes, A.; Klanner, R.; Kogler, R.; Lapsien, T.; Lenz, T.; Marchesini, I.; Marconi, D.; Nowatschin, D.; Ott, J.; Pantaleo, F.; Peiffer, T.; Perieanu, A.; Pietsch, N.; Poehlsen, J.; Rathjens, D.; Sander, C.; Schettler, H.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Schwandt, J.; Seidel, M.; Sola, V.; Stadie, H.; Steinbrueck, G.; Tholen, H.; Troendle, D.; Usai, E.; Vanelderen, L.; Vanhoefer, A.; Andreev, V.; Azzolini, V.] Univ Hamburg, Hamburg, Germany. [Akbiyik, M.; Amstutz, C.; Barth, C.; Baus, C.; Berger, J.; Beskidt, C.; Boeser, C.; Butz, E.; Caspart, R.; Chwalek, T.; Colombo, F.; De Boer, W.; Descroix, A.; Dierlamm, A.; Eber, R.; Feindt, M.; Fink, S.; Fischer, M.; Frensch, F.; Freund, B.; Friese, R.; Funke, D.; Giffels, M.; Gilbert, A.; Haitz, D.; Harbaum, T.; Harrendorf, M. A.; Hartmann, F.; Husemann, U.; Kassel, F.; Katkov, I.; Kornmayer, A.; Kudella, S.; Pardo, P. Lobelle; Maier, B.; Mildner, H.; Mozer, M. U.; Mueller, T.; Mueller, Th.; Plagge, M.; Printz, M.; Quast, G.; Rabbertz, K.; Roecker, S.; Roscher, F.; Shvetsov, I.; Sieber, G.; Simonis, H. J.; Stober, F. M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weiler, T.; Williamson, S.; Woehrmann, C.; Wolf, R.] Univ Karlsruhe, Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Giakoumopoulou, V. A.; Kyriakis, A.; Loukas, D.; Markou, A.; Psallidas, A.; Topsis-Giotis, I.] NCSR Demokritos, Inst Nucl & Particle Phys, Aghia Paraskevi, Greece. [Agapitos, A.; Kesisoglou, S.; Panagiotou, A.; Saoulidou, N.; Tziaferi, E.] Univ Athens, Athens, Greece. [Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Loukas, N.; Manthos, N.; Papadopoulos, I.; Paradas, E.; Strologas, J.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hazi, A.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.] Wigner Res Ctr Phys, Budapest, Hungary. [Horvath, D.; Beni, N.; Czellar, S.; Karancsi, J.; Molnar, J.; Szillasi, Z.; Yi, K.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Karancsi, J.; Bartok, M.; Makovec, A.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, Debrecen, Hungary. [Mal, P.; Mandal, K.; Sahoo, N.; Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Bansal, S.; Beri, S. B.; Bhatnagar, V.; Chawla, R.; Gupta, R.; Bhawandeep, U.; Kalsi, A. K.; Kaur, A.; Kaur, M.; Kumar, R.; Mehta, A.; Mittal, M.; Nishu, N.; Singh, J. B.; Walia, G.] Panjab Univ, Chandigarh 160014, India. [Kumar, Ashok; Kumar, Arun; Bhardwaj, A.; Choudhary, B. C.; Garg, R. B.; Kumar, A.; Malhotra, S.; Naimuddin, M.; Ranjan, K.; Sharma, R.; Sharma, V.] Univ Delhi, Delhi 110007, India. [Banerjee, S.; Bhattacharya, S.; Chatterjee, K.; Dey, S.; Dutta, S.; Jain, Sa.; Jain, Sh.; Khurana, R.; Majumdar, N.; Modak, A.; Mondal, K.; Mukherjee, S.; Mukhopadhyay, S.; Roy, A.; Roy, D.; Chowdhury, S. Roy; Sarkar, S.; Sharan, M.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Chudasama, R.; Dutta, D.; Jha, V.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Bombay 400085, Maharashtra, India. [Aziz, T.; Banerjee, S.; Bhowmik, S.; Chatterjee, R. M.; Dewanjee, R. K.; Dugad, S.; Ganguly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Kole, G.; Kumar, S.; Mahakud, B.; Maity, M.; Majumder, G.; Mazumdar, K.; Mitra, S.; Mohanty, G. B.; Parida, B.; Sarkar, T.; Sudhakar, K.; Sur, N.; Sutar, B.; Wickramage, N.] Tata Inst Fundamental Res, Homi Bhabha Rd, Bombay 400005, Maharashtra, India. [Sharma, S.] Indian Inst Sci Educ & Res, Pune, Maharashtra, India. [Bakhshiansohi, H.; Behnamian, H.; Etesami, S. M.; Fahim, A.; Goldouzian, R.; Khakzad, M.; Najafabadi, M. Mohammadi; Naseri, M.; Mehdiabadi, S. Paktinat; Hosseinabadi, F. Rezaei; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Felcini, M.; Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Abbrescia, M.; Calabria, C.; Caputo, C.; Chhibra, S. S.; Colaleo, A.; Creanza, D.; Cristella, L.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; Miniello, G.; My, S.; Nuzzo, S.; Pompili, A.; Pugliese, G.; Radogna, R.; Ranieri, A.; Selvaggi, G.; Silvestris, L.; Venditti, R.; Verwilligen, P.; Andreev, V.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Abbrescia, M.; Calabria, C.; Caputo, C.; Chhibra, S. S.; Cristella, L.; De Palma, M.; Miniello, G.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Battilana, C.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Montanari, A.; Navarria, F. L.; Perrotta, A.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Navarria, F. L.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Cappello, G.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Chiorboli, M.; Costa, S.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. CSFNSM, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.; Viliani, L.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.; Viliani, L.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Fabbri, F.; Piccolo, D.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Calvelli, V.; Ferro, F.; Lo Vetere, M.; Robutti, E.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, Via Dodecaneso 33, I-16146 Genoa, Italy. [Calvelli, V.; Lo Vetere, M.; Tosi, S.] Univ Genoa, Genoa, Italy. [Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Malvezzi, S.; Manzoni, R. A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; Fatis, T. Tabarelli de] Ist Nazl Fis Nucl, Sez Milano Bicocca, Via Celoria 16, I-20133 Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Manzoni, R. A.; Marzocchi, B.; Paganoni, M.; Ragazzi, S.; Fatis, T. Tabarelli de] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Di Guida, S.; Esposito, M.; Fabozzi, F.; Iorio, A. O. M.; Lanza, G.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.; Sciacca, C.; Thyssen, F.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Buontempo, S.; Cavallo, N.; Di Guida, S.; Esposito, M.; Fabozzi, F.; Iorio, A. O. M.; Lanza, G.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.; Sciacca, C.; Thyssen, F.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Esposito, M.; Iorio, A. O. M.; Sciacca, C.] Univ Naples Federico II, Naples, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata, I-85100 Potenza, Italy. [Di Guida, S.; Meola, S.] Univ G Marconi, Rome, Italy. [Azzi, P.; Bacchetta, N.; Bisello, D.; Branca, A.; Carlin, R.; De Oliveira, A. Carvalho Antunes; Checchia, P.; Dall'Osso, M.; Dorigo, T.; Dosselli, U.; Gasparini, F.; Gasparini, U.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Simonetto, F.; Torassa, E.; Tosi, M.; Ventura, S.; Zanetti, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.; Andreev, V.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Bisello, D.; Branca, A.; Carlin, R.; De Oliveira, A. Carvalho Antunes; Dall'Osso, M.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.] Univ Trento, Trento, Italy. [Braghieri, A.; Gabusi, M.; Magnani, A.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vai, I.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Gabusi, M.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, Via Palestro 3, I-27100 Pavia, Italy. [Solestizi, L. Alunni; Biasini, M.; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Solestizi, L. Alunni; Biasini, M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Fedi, G.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.; Barone, L.; Andreev, V.; Rolandi, G.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; Donato, S.; Foa, L.; Ligabue, F.; Rolandi, G.] Scuola Normale Super Pisa, Pisa, Italy. [Cavallari, F.; D'imperio, G.; Del Re, D.; Diemoz, M.; Gelli, S.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Micheli, F.; Organtini, G.; Paramatti, R.; Preiato, F.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Traczyk, P.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [D'imperio, G.; Del Re, D.; Longo, E.; Margaroli, F.; Micheli, F.; Organtini, G.; Preiato, F.; Rahatlou, S.; Santanastasio, F.; Traczyk, P.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Costa, M.; Covarelli, R.; De Remigis, P.; Degano, A.; Demaria, N.; Finco, L.; Mariotti, C.; Maselli, S.; Mazza, G.; Migliore, E.; Monaco, V.; Monteil, E.; Musich, M.; Obertino, M. M.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Andreev, V.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Costa, M.; Covarelli, R.; Degano, A.; Finco, L.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Ruspa, M.] Univ Piemonte Orientale, Novara, Italy. [Belforte, S.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Schizzi, A.; Umer, T.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Schizzi, A.; Umer, T.] Univ Trieste, Trieste, Italy. [Chang, S.; Kropivnitskaya, A.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Sakharov, A.; Son, D. C.; Kamon, T.] Kyungpook Natl Univ, Daegu, South Korea. [Cifuentes, J. A. Brochero; Kim, H.; Kim, T. J.; Ryu, M. S.] Chonbuk Natl Univ, Jeonju 561756, South Korea. [Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Choi, S.; Go, Y.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, Y.; Lee, B.; Lee, K.; Lee, K. S.; Lee, S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Yoo, H. D.] Seoul Natl Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Lee, J. S. H.; Park, I. C.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Choi, Y. K.; Goh, J.; Kim, D.; Kwon, E.; Lee, J.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.; Vaitkus, J.] Vilnius State Univ, Vilnius, Lithuania. [Ahmed, I.; Ibrahim, Z. A.; Komaragiri, J. R.; Ali, M. A. B. Md; Idris, F. Mohamad; Abdullah, W. A. T. Wan] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Casimiro Linares, E.; Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Hernandez-Almada, A.; Lopez-Fernandez, R.; Sanchez-Hernandez, A.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Carpinteyro, S.; Pedraza, I.; Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.; Reucroft, S.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, A.; Ahmad, M.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.; Walczak, M.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz E Silva, C.; Di Francesco, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Lloret Iglesias, L.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Toldaiev, O.; Vadruccio, D.; Varela, J.; Vischia, P.; Yi, K.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Finger, M.; Tsamalaidze, Z.; Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Shulha, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Kuznetsova, E.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Matveev, V.; Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Karneyeu, A.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Pozdnyakov, I.; Safronov, G.; Spiridonov, A.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Bylinkin, A.; Azarkin, M.; Dremin, I.; Leonidov, A.] Natl Res Nucl Univ, Moscow Engn Phys Inst MEPhI, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Leninsky Prospect 53, Moscow 117924, Russia. [Popov, A.; Zhukov, V.; Katkov, I.; Baskakov, A.; Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Myagkov, I.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia. [Adzic, P.; Ekmedzic; Milosevic, J.; Rekovic, V.; Milenovic, P.] Univ Belgrade, Fac Phys, POB 550, Belgrade 11001, Serbia. [Adzic, P.; Ekmedzic; Milosevic, J.; Rekovic, V.; Milenovic, P.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia. [Alcaraz Maestre, J.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.] CIEMAT, E-28040 Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Brun, H.; Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Palencia Cortezon, E.; Vizan Garcia, J. M.] Univ Oviedo, Oviedo, Spain. [Cabrillo, I. J.; Calderon, A.; Castineiras De Saa, J. R.; Duarte Campderros, J.; Fernandez, M.; Gomez, G.; Graziano, A.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Rabady, D.; Genchev, V.; Merlin, J. A.; Lingemann, J.; Pantaleo, F.; Hartmann, F.; Kassel, F.; Kornmayer, A.; Mohanty, A. K.; Fahim, A.; Silvestris, L.; Battilana, C.; Marzocchi, B.; Di Guida, S.; Meola, S.; Paolucci, P.; Azzi, P.; Dall'Osso, M.; Zucchetta, A.; Ciangottini, D.; Donato, S.; D'imperio, G.; Traczyk, P.; Finco, L.; Candelise, V.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Berruti, G. M.; Bianchi, G.; Bloch, P.; Bocci, A.; Bonato, A.; Botta, C.; Breuker, H.; Camporesi, T.; Cerminara, G.; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; Daponte, V.; David, A.; De Gruttola, M.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Marco, E.; Dobson, M.; Dordevic, M.; du Pree, T.; Dupont, N.; Elliott-Peisert, A.; Eugster, J.; Franzoni, G.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Hansen, M.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kirschenmann, H.; Kortelainen, M. J.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Lucchini, M. T.; Magini, N.; Malgeri, L.; Mannelli, M.; Marrouche, J.; Martelli, A.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Nemallapudi, M. V.; Neugebauer, H.; Orfanelli, S.; Orsini, L.; Pape, L.; Perez, E.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Piparo, D.; Racz, A.; Rolandi, G.; Rovere, M.; Ruan, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Sharma, A.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Steggemann, J.; Stieger, B.; Stoye, M.; Takahashi, Y.; Treille, D.; Tsirou, A.; Veres, G. I.; Wardle, N.; Woehri, H. K.; Zagozdzinska, A.; Zeuner, W. D.; Ulmer, K. A.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Buchmann, M. A.; Casal, B.; Dissertori, G.; Dittmar, M.; Donega, M.; Duenser, M.; Eller, P.; Grab, C.; Heidegger, C.; Hits, D.; Hoss, J.; Kasieczka, G.; Lustermann, W.; Marini, A. C.; Marionneau, M.; del Arbol, P. Martinez Ruiz; Masciovecchio, M.; Meister, D.; Musella, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pata, J.; Pauss, F.; Perrozzi, L.; Peruzzi, M.; Quittnat, M.; Rossini, M.; Starodumov, A.; Takahashi, M.; Tavolaro, V. R.; Theofilatos, K.; Wallny, R.; Weber, H. A.] Swiss Fed Inst Technol, Inst Particle Phys, Zurich, Switzerland. [Aarrestad, T. K.; Amsler, C.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Galloni, C.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Ngadiuba, J.; Pinna, D.; Robmann, P.; Ronga, F. J.; Salerno, D.; Taroni, S.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Doan, T. H.; Ferro, C.; Konyushikhin, M.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Volpe, R.; Yu, S. S.] Natl Cent Univ, Chungli, Taiwan. [Bartek, R.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Fiori, F.; Grundler, U.; Hou, W-S; Hsiung, Y.; Kao, K. Y.; Liu, Y. F.; Lu, R-S; Moya, M. Minano; Petrakou, E.; Tsai, J. F.; Tzeng, Y. M.; Majumder, D.] Natl Taiwan Univ NTU, Taipei, Taiwan. [Asavapibhop, B.; Kovitanggoon, K.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Dept Phys, Fac Sci, Bangkok, Thailand. [Adiguzel, A.; Cerci, S.; Dozen, C.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Tali, B.; Topakli, H.; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Isildak, B.; Karapinar, G.; Surat, U. E.; Yalvac, M.; Zeyrek, M.; Albayrak, E. A.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Kaya, M.; Kaya, O.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cankocak, K.; Sen, S.; Vardarli, F. I.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Grynyov, B.] Natl Acad Sci Ukraine, Inst Scintillat Mat, Kharkov, Ukraine. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Aggleton, R.; Ball, F.; Beck, L.; Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Sakuma, T.; El Nasr-storey, S. Seif; Senkin, S.; Smith, D.; Smith, V. J.] Univ Bristol, Bristol, Avon, England. [Newbold, D. M.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Thomas, L.; Tomalin, I. R.; Williams, T.; Womersley, W. J.; Worm, S. D.; Baber, M.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Bainbridge, R.; Buchmuller, O.; Bundock, A.; Burton, D.; Casasso, S.; Citron, M.; Colling, D.; Corpe, L.; Cripps, N.; Dauncey, P.; Davies, G.; De Wit, A.; Della Negra, M.; Dunne, P.; Elwood, A.; Ferguson, W.; Fulcher, J.; Futyan, D.; Hall, G.; Iles, G.; Karapostoli, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A-M; Malik, S.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Richards, A.; Rose, A.; Seez, C.; Sharp, P.; Tapper, A.; Uchida, K.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Borzou, A.; Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Pastika, N.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Gastler, D.; Lawson, P.; Rankin, D.; Richardson, C.; Rohlf, J.; St John, J.; Sulak, L.; Zou, D.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Berry, E.; Bhattacharya, S.; Cutts, D.; Dhingra, N.; Ferapontov, A.; Garabedian, A.; Heintz, U.; Laird, E.; Landsberg, G.; Mao, Z.; Narain, M.; Sagir, S.; Sinthuprasith, T.] Brown Univ, Providence, RI 02912 USA. [Shulha, S.; Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Lander, R.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.; Yi, K.] Univ Calif Davis, Davis, CA 95616 USA. [Cousins, R.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Rakness, G.; Saltzberg, D.; Takasugi, E.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Paneva, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Negrete, M. Olmedo; Shrinivas, A.; Sumowidagdo, S.; Wei, H.; Wimpenny, S.] Univ Calif Riverside, Riverside, CA 92521 USA. [Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Holzner, A.; Kelley, R.; Klein, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Tadel, M.; Tu, Y.; Vartak, A.; Wasserbaech, S.; Welke, C.; Wuerthwein, F.; Yagil, A.; Della Porta, G. Zevi] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bradmiller-Feld, J.; Campagnari, C.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Gran, J.; Incandela, J.; Justus, C.; Mccoll, N.; Mullin, S. D.; Richman, J.; Stuart, D.; Suarez, I.; To, W.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dubinin, M.; Anderson, D.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Pierini, M.; Spiropulu, M.; Vlimant, J. R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Iiyama, Y.; Paulini, M.; Russ, J.; Sun, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Jensen, F.; Johnson, A.; Krohn, M.; Mulholland, T.; Nauenberg, U.; Smith, J. G.; Stenson, K.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Rinkevicius, A.; Ryd, A.; Skinnari, L.; Soffi, L.; Sun, W.; Tan, S. M.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Aleksandrov, A.; Avetisyan, A.; Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hooberman, B.; Hu, Z.; Jindariani, S.; Johnson, M.; Joshi, U.; Jung, A. W.; Klima, B.; Kreis, B.; Kwan, S.; Lammel, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; De Sa, R. Lopes; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mishra, K.; Mrenna, S.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Prokofyev, O.; Sexton-Kennedy, E.; Soha, A.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vernieri, C.; Verzocchi, M.; Vidal, R.; Whitbeck, A.; Yang, F.; Yin, H.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Carnes, A.; Carver, M.; Curry, D.; Das, S.; Di Giovanni, G. P.; Field, R. D.; Fisher, M.; Furic, I. K.; Hugon, J.; Konigsberg, J.; Korytov, A.; Low, J. F.; Ma, P.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Muniz, L.; Rank, D.; Shchutska, L.; Snowball, M.; Sperka, D.; Wang, S.; Yelton, J.] Univ Florida, Gainesville, FL USA. [Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Ackert, A.; Adams, J. R.; Adams, T.; Askew, A.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Jenkins, M.; Johnson, K. F.; Khatiwada, A.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Bhopatkar, V.; Hohlmann, M.; Kalakhety, H.; Mareskas-Palcek, D.; Roy, T.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Berry, D.; Betts, R. 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[Chakaberia, I.; Ivanov, A.; Kaadze, K.; Khalil, S.; Makouski, M.; Maravin, Y.; Saini, L. K.; Skhirtladze, N.; Svintradze, I.; Toda, S.] Kansas State Univ, Manhattan, KS 66506 USA. [Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Anelli, C.; Baden, A.; Baron, O.; Belloni, A.; Calvert, B.; Eno, S. C.; Ferraioli, C.; Gomez, J. A.; Hadley, N. J.; Jabeen, S.; Kellogg, R. G.; Kolberg, T.; Kunkle, J.; Lu, Y.; Mignerey, A. C.; Pedro, K.; Shin, Y. H.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Baty, A.; Bierwagen, K.; Brandt, S.; Busza, W.; Cali, I. A.; Demiragli, Z.; Di Matteo, L.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Innocenti, G. M.; Klute, M.; Kovalskyi, D.; Lai, Y. S.; Lee, Y-J; Levin, A.; Luckey, P. D.; Mcginn, C.; Niu, X.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Stephans, G. S. F.; Sumorok, K.; Varma, M.; Velicanu, D.; Veverka, J.; Wang, J.; Wang, T. 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A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Palmer, C.; Piroue, P.; Quan, X.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Malik, S.] Univ Puerto Rico, Mayaguez, PR USA. [Savoy-Navarro, A.; Venturi, A.; Barnes, V. E.; Benedetti, D.; Bortoletto, D.; Gutay, L.; Jha, M. K.; Jones, M.; Jung, K.; Kress, M.; Leonardo, N.; Miller, D. H.; Neumeister, N.; Primavera, F.; Radburn-Smith, B. C.; Shi, X.; Shipsey, I.; Silvers, D.; Sun, J.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.; Zablocki, J.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.; Stupak, J.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Chen, Z.; Ecklund, K. M.; Geurts, F. J. M.; Guilbaud, M.; Li, W.; Michlin, B.; Northup, M.; Padley, B. P.; Redjimi, R.; Roberts, J.; Rorie, J.; Tu, Z.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Galanti, M.; Garcia-Bellido, A.; Goldenzweig, P.; Han, J.; Harel, A.; Hindrichs, O.; Khukhunaishvili, A.; Petrillo, G.; Verzetti, M.] Univ Rochester, Rochester, NY 14627 USA. [Demortier, L.] Rockefeller Univ, 1230 York Ave, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Hughes, E.; Kaplan, S.; Elayavalli, R. Kunnawalkam; Lath, A.; Panwalkar, S.; Park, M.; Salur, S.; Schnetzer, S.; Sheffield, D.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Foerster, M.; Riley, G.; Rose, K.; Spanier, S.; York, A.] Univ Tennessee, Knoxville, TN USA. [Bouhali, O.; Hernandez, A. 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[Kaya, O.] Kafkas Univ, Kars, Turkey. [Yetkin, T.] Yildiz Tech Univ, Istanbul, Turkey. [Sen, S.] Hacettepe Univ, Ankara, Turkey. [Belyaev, A.; Kenny, R. P., III] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Acosta, M. Vazquez] Inst Astrofis Canarias, E-38200 San Cristobal la Laguna, Spain. [Wasserbaech, S.] Utah Valley Univ, Orem, UT USA. [Bilki, B.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Bouhali, O.] Texas A&M Univ Qatar, Doha, Qatar. RP Khachatryan, V (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Calderon, Alicia/K-3658-2014; Goh, Junghwan/Q-3720-2016; Flix, Josep/G-5414-2012; Nguyen, Federico/Q-8994-2016; Ruiz, Alberto/E-4473-2011; Petrushanko, Sergey/D-6880-2012; Dudko, Lev/D-7127-2012; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Leonidov, Andrey/M-4440-2013; Paulini, Manfred/N-7794-2014; Smirnov, Vitaly/B-5001-2017; Mora Herrera, Maria Clemencia/L-3893-2016; Mundim, Luiz/A-1291-2012; Colafranceschi, Stefano/M-1807-2016; TUVE', Cristina/P-3933-2015; Raidal, Martti/F-4436-2012; Konecki, Marcin/G-4164-2015; Vogel, Helmut/N-8882-2014; Benussi, Luigi/O-9684-2014; Andreev, Vladimir/M-8665-2015; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Della Ricca, Giuseppe/B-6826-2013; Stahl, Achim/E-8846-2011; Manganote, Edmilson/K-8251-2013; Lokhtin, Igor/D-7004-2012; VARDARLI, Fuat Ilkehan/B-6360-2013; Varela, Joao/K-4829-2016; Seixas, Joao/F-5441-2013; Verwilligen, Piet/M-2968-2014; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Da Silveira, Gustavo Gil/N-7279-2014; Moraes, Arthur/F-6478-2010; Ogul, Hasan/S-7951-2016; Dremin, Igor/K-8053-2015; Azarkin, Maxim/N-2578-2015; ciocci, maria agnese /I-2153-2015; Kirakosyan, Martin/N-2701-2015; Puljak, Ivica/D-8917-2017; OI Goh, Junghwan/0000-0002-1129-2083; Flix, Josep/0000-0003-2688-8047; Nguyen, Federico/0000-0002-6713-1596; Ruiz, Alberto/0000-0002-3639-0368; Dudko, Lev/0000-0002-4462-3192; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Mundim, Luiz/0000-0001-9964-7805; TUVE', Cristina/0000-0003-0739-3153; Konecki, Marcin/0000-0001-9482-4841; Vogel, Helmut/0000-0002-6109-3023; Benussi, Luigi/0000-0002-2363-8889; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Della Ricca, Giuseppe/0000-0003-2831-6982; Stahl, Achim/0000-0002-8369-7506; Varela, Joao/0000-0003-2613-3146; Seixas, Joao/0000-0002-7531-0842; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Moraes, Arthur/0000-0002-5157-5686; Ogul, Hasan/0000-0002-5121-2893; ciocci, maria agnese /0000-0003-0002-5462; Androsov, Konstantin/0000-0003-2694-6542; Viliani, Lorenzo/0000-0002-1909-6343; ROMERO ABAD, DAVID/0000-0001-5088-9301; Gallinaro, Michele/0000-0003-1261-2277 FU Austrian Federal Ministry of Science; Research and Economy; Austrian Science Fund; Belgian Fonds de la Recherche Scientifique and Fonds voor Wetenschappelijk Onderzoek; Brazilian Funding Agency (CNPq); Brazilian Funding Agency (CAPES); Brazilian Funding Agency (FAPERJ); Brazilian Funding Agency (FAPESP); Bulgarian Ministry of Education and Science; CERN; Chinese Academy of Sciences; Ministry of Science and Technology; National Natural Science Foundation of China; Colombian Funding Agency (COLCIENCIAS); Croatian Ministry of Science, Education and Sport; Croatian Science Foundation; Research Promotion Foundation, Cyprus; Ministry of Education and Research, Estonian Research Council [IUT23-4, IUT23-6]; European Regional Development Fund, Estonia; Academy of Finland; Finnish Ministry of Education and Culture; Helsinki Institute of Physics; Institut National de Physique Nucleaire et de Physique des Particules/CNRS; Commissariat a l'Energie Atomique et aux Energies Alternatives/CEA, France; Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft, Germany; Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; General Secretariat for Research and Technology, Greece; National Scientific Research Foundation, Hungary; National Innovation Office, Hungary; Department of Atomic Energy, India; Department of Science and Technology, India; Institute for Studies in Theoretical Physics and Mathematics, Iran; Science Foundation, Ireland; Istituto Nazionale di Fisica Nucleare, Italy; Ministry of Science, ICT and Future Planning; National Research Foundation, Republic of Korea; Lithuanian Academy of Sciences; Ministry of Education, and University of Malaya (Malaysia); Mexican Funding Agency (CINVESTAV); Mexican Funding Agency (CONACYT); Mexican Funding Agency (SEP); Mexican Funding Agency (UASLP-FAI); Ministry of Business, Innovation and Employment, New Zealand; Pakistan Atomic Energy Commission; Ministry of Science and Higher Education, Poland; National Science Centre, Poland; Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; Ministry of Education and Science of the Russian Federation; Federal Agency of Atomic Energy of the Russian Federation; Russian Academy of Sciences; Russian Foundation for Basic Research; Ministry of Education, Science and Technological Development of Serbia; Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio, Spain; Swiss Funding Agency (ETH Board); Swiss Funding Agency (ETH Zurich); Swiss Funding Agency (PSI); Swiss Funding Agency (SNF); Swiss Funding Agency (UniZH); Swiss Funding Agency (Canton Zurich); Swiss Funding Agency (SER); Ministry of Science and Technology, Taipei; Thailand Center of Excellence in Physics; Institute for the Promotion of Teaching Science and Technology of Thailand; Special Task Force for Activating Research; National Science and Technology Development Agency of Thailand; Scientific and Technical Research Council of Turkey and Turkish Atomic Energy Authority; National Academy of Sciences of Ukraine and State Fund for Fundamental Researches, Ukraine; Science and Technology Facilities Council, UK; US Department of Energy; US National Science Foundation; Marie-Curie program; European Research Council and EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (Belgium); Ministry of Education; Youth and Sports of the Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS program of the Foundation for Polish Science; European Union; Regional Development Fund; Compagnia di San Paolo (Torino); Consorzio per la Fisica (Trieste); MIUR Project (Italy) [20108T4XTM]; Thalis and Aristeia programs - EU-ESF; Greek NSRF; National Priorities Research Program by Qatar National Research Fund; Rachadapisek Sompot Fund for Postdoctoral Fellowship; Chulalongkorn University (Thailand); Welch Foundation FX Bundes-ministerium Forschungs-gemeinschaft Forschungs-zentren We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses.; Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: the Austrian Federal Ministry of Science, Research and Economy and the Austrian Science Fund; the Belgian Fonds de la Recherche Scientifique and Fonds voor Wetenschappelijk Onderzoek; the Brazilian Funding Agencies (CNPq, CAPES, FAPERJ, and FAPESP); the Bulgarian Ministry of Education and Science; CERN; the Chinese Academy of Sciences, Ministry of Science and Technology, and National Natural Science Foundation of China; the Colombian Funding Agency (COLCIENCIAS); the Croatian Ministry of Science, Education and Sport and the Croatian Science Foundation; the Research Promotion Foundation, Cyprus; the Ministry of Education and Research, Estonian Research Council via IUT23-4 and IUT23-6 and European Regional Development Fund, Estonia; the Academy of Finland, Finnish Ministry of Education and Culture, and Helsinki Institute of Physics; the Institut National de Physique Nucleaire et de Physique des Particules/CNRS and Commissariat a l'Energie Atomique et aux Energies Alternatives/CEA, France; the Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft and Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; the General Secretariat for Research and Technology, Greece; the National Scientific Research Foundation and National Innovation Office, Hungary; the Department of Atomic Energy and the Department of Science and Technology, India; the Institute for Studies in Theoretical Physics and Mathematics, Iran; the Science Foundation, Ireland; the Istituto Nazionale di Fisica Nucleare, Italy; the Ministry of Science, ICT and Future Planning, and National Research Foundation, Republic of Korea; the Lithuanian Academy of Sciences; the Ministry of Education, and University of Malaya (Malaysia); the Mexican Funding Agencies (CINVESTAV, CONACYT, SEP, and UASLP-FAI); the Ministry of Business, Innovation and Employment, New Zealand; the Pakistan Atomic Energy Commission; the Ministry of Science and Higher Education and the National Science Centre, Poland; the Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; the Ministry of Education and Science of the Russian Federation, the Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences, and the Russian Foundation for Basic Research; the Ministry of Education, Science and Technological Development of Serbia; the Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio 2010, Spain; the Swiss Funding Agencies (ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER); the Ministry of Science and Technology, Taipei; the Thailand Center of Excellence in Physics, the Institute for the Promotion of Teaching Science and Technology of Thailand, Special Task Force for Activating Research and the National Science and Technology Development Agency of Thailand; the Scientific and Technical Research Council of Turkey and Turkish Atomic Energy Authority; the National Academy of Sciences of Ukraine and State Fund for Fundamental Researches, Ukraine; the Science and Technology Facilities Council, UK; the US Department of Energy and the US National Science Foundation. Individuals have received support from the Marie-Curie program and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P.; Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (Belgium); the Ministry of Education, Youth and Sports of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS program of the Foundation for Polish Science, cofinanced from European Union, Regional Development Fund; the Compagnia di San Paolo (Torino); the Consorzio per la Fisica (Trieste); MIUR Project No. 20108T4XTM (Italy); the Thalis and Aristeia programs cofinanced by EU-ESF and the Greek NSRF; the National Priorities Research Program by Qatar National Research Fund; the Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); and the Welch Foundation. NR 59 TC 5 Z9 5 U1 19 U2 39 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JUN 15 PY 2016 VL 93 IS 11 AR 112009 DI 10.1103/PhysRevD.93.112009 PG 32 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DO5DZ UT WOS:000377805100001 ER PT J AU Lind, KR Lee, N Sizmur, T Siemianowski, O Van Bruggen, S Ganapathysubramaniam, B Cademartiri, L AF Lind, Kara R. Lee, Nigel Sizmur, Tom Siemianowski, Oskar Van Bruggen, Shawn Ganapathysubramaniam, Baskar Cademartiri, Ludovico TI Plant Growth Environments with Programmable Relative Humidity and Homogeneous Nutrient Availability SO PLOS ONE LA English DT Article ID PHENOMICS; TECHNOLOGIES; HYPOTHESIS; RESPONSES; HISTORY; FUTURE; LIFE AB We describe the design, characterization, and use of "programmable", sterile growth environments for individual (or small sets of) plants. The specific relative humidities and nutrient availability experienced by the plant is established (RH between 15% and 95%; nutrient concentration as desired) during the setup of the growth environment, which takes about 5 minutes and < 1$ in disposable cost. These systems maintain these environmental parameters constant for at least 14 days with minimal intervention (one minute every two days). The design is composed entirely of off-the-shelf components (e.g., LEGO1 bricks) and is characterized by (i) a separation of root and shoot environment (which is physiologically relevant and facilitates imposing specific conditions on the root system, e.g., darkness), (ii) the development of the root system on a flat surface, where the root enjoys constant contact with nutrient solution and air, (iii) a compatibility with root phenotyping. We demonstrate phenotyping by characterizing root systems of Brassica rapa plants growing in different relative humidities (55%, 75%, and 95%). While most phenotypes were found to be sensitive to these environmental changes, a phenotype tightly associated with root system topology-the size distribution of the areas encircled by roots-appeared to be remarkably and counter-intuitively insensitive to humidity changes. These setups combine many of the advantages of hydroponics conditions (e.g., root phenotyping, complete control over nutrient composition, scalability) and soil conditions (e.g., aeration of roots, shading of roots), while being comparable in cost and setup time to Magenta (R) boxes. C1 [Lind, Kara R.; Sizmur, Tom; Siemianowski, Oskar; Cademartiri, Ludovico] Iowa State Univ Sci & Technol, Dept Mat Sci & Engn, Ames, IA 50011 USA. [Lee, Nigel; Ganapathysubramaniam, Baskar] Iowa State Univ Sci & Technol, Dept Mech Engn, Ames, IA 50011 USA. [Sizmur, Tom] Univ Reading, Dept Geog & Environm Sci, Reading, Berks, England. [Van Bruggen, Shawn; Cademartiri, Ludovico] Iowa State Univ Sci & Technol, Dept Chem & Biol Engn, Ames, IA 50011 USA. [Sizmur, Tom; Cademartiri, Ludovico] US DOE, Ames Lab, Ames, IA 50011 USA. RP Cademartiri, L (reprint author), Iowa State Univ Sci & Technol, Dept Mat Sci & Engn, Ames, IA 50011 USA.; Cademartiri, L (reprint author), Iowa State Univ Sci & Technol, Dept Chem & Biol Engn, Ames, IA 50011 USA.; Cademartiri, L (reprint author), US DOE, Ames Lab, Ames, IA 50011 USA. EM lcademar@iastate.edu RI Cademartiri, Ludovico/A-4142-2008 OI Cademartiri, Ludovico/0000-0001-8805-9434 FU Arnold and Mabel Beckman Foundation; Plant Science Institute at Iowa State University FX The work was funded by the Arnold and Mabel Beckman Foundation through a Young Investigator Award to LC. Root phenotyping work was separately funded by the Plant Science Institute at Iowa State University through a Faculty Scholar Award to LC. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 32 TC 0 Z9 0 U1 10 U2 14 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD JUN 15 PY 2016 VL 11 IS 6 AR e0155960 DI 10.1371/journal.pone.0155960 PG 15 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DO5LO UT WOS:000377824800011 PM 27304431 ER PT J AU Yi, XO Jenkins, ML Kirk, MA Zhou, ZF Roberts, SG AF Yi, Xiaoou Jenkins, Michael L. Kirk, Marquis A. Zhou, Zhongfu Roberts, Steven G. TI In-situ TEM studies of 150 keV W+ ion irradiated W and W-alloys: Damage production and microstructural evolution SO ACTA MATERIALIA LA English DT Article DE W/W-alloys; In-situ irradiations; TEM; Damage production; Microstructure evolution ID FE-CR ALLOYS; DISLOCATION LOOPS; NEUTRON-IRRADIATION; RADIATION-DAMAGE; SPATIAL-DISTRIBUTION; COLLISION CASCADES; PRIMARY STATE; THIN-FOILS; TUNGSTEN; DEFECTS AB In-situ irradiations with 150 keV W+ ions have been performed on W and W-5wt.% (Re; Ta; V) alloys in a comprehensive study of the influences of irradiation temperature T-irr, dose, alloying elements and grain orientations on radiation damage production and microstructural evolution. For T-irr between 30 K and 1073 K, the first observable defects in pure W appeared at doses <= 0.01 dpa, and were most likely vacancy loops, with Burgers vectors predominantly of type b = 1/2 < 111 >. With increasing T-irr, the retained defect concentration decreased strongly and the maximum cluster size increased from similar to 1300 point defects at 30 K to similar to 2300 point defects at 1073 K. At all irradiation temperatures, the evolution of damage microstructures with dose from 0.1 to 1.0 dpa involved defect cluster migration, with mutual elastic interactions often leading to spatial inhomogeneities and loop reactions. In pure W, spatial ordering of loops was observed at doses >0.4 dpa and T-irr >= 773 K in grains close to z = < 001 >. No such ordering was found in similar grain orientations for the W-(Re; Ta) alloys, but it was found in the non-z = < 001 > grains. Post-irradiation analysis on W and W-5 wt% (Re; Ta) at 1.0 dpa showed that 1/2 < 111 > and < 100 > loops of both vacancy and interstitial type were present, at number densities similar to 10(15) loops m(-2). In all cases 1/2 < 111 > loops were dominant, the fraction of these with interstitial nature increased with T-irr, and the proportion of < 100 > loops decreased with increasing T-irr. Compared with pure W, microstructures in the W-(Re; Ta) alloys exhibited higher loop number densities and evolved more quickly with increasing dose towards damage saturation. (C) 2016 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Yi, Xiaoou] Univ Sci & Technol Beijing, Sch Mat Sci & Engn, Beijing 100083, Peoples R China. [Jenkins, Michael L.] Univ Oxford, Trinity Coll, Broad St, Oxford OX1 3BH, England. [Kirk, Marquis A.] Argonne Natl Lab, Nucl Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Zhou, Zhongfu] Shanghai Univ, Key Lab Mat Microstruct, Shanghai 200444, Peoples R China. [Zhou, Zhongfu] Aberystwyth Univ, Inst Math & Phys, Aberystwyth SY23 3BZ, Dyfed, Wales. [Roberts, Steven G.] Univ Oxford, Dept Mat, Parks Rd, Oxford OX1 3PH, England. [Roberts, Steven G.] Culham Sci Ctr, CCFE, Abingdon OX14 3DB, Oxon, England. RP Yi, XO (reprint author), Univ Sci & Technol Beijing, Sch Mat Sci & Engn, Beijing 100083, Peoples R China. EM xiaoouyi@ustb.edu.cn FU DOE Office of Nuclear Energy [DE-AC02-06CH11357]; Culham Centre for Fusion Energy, St Edmund Hall, University of Oxford; EPSRC [EP/H018921/1] FX The electron microscopy with in-situ ion irradiation was carried out at Argonne National Laboratory at the IVEM-Tandem Facility, a U.S. Department of Energy Facility funded by the DOE Office of Nuclear Energy, operated under Contract No. DE-AC02-06CH11357 by UChicago Argonne, LLC. We thank Pete Baldo and Edward Ryan for their help with the irradiations. XY thanks Prof. Sergei Dudarev, Dr. Daniel Mason, Dr. Duc Nguyen-Manh and Dr. Mark Gilbert for fruitful discussions, and the Culham Centre for Fusion Energy for funding via a Junior Research Fellowship at St Edmund Hall, University of Oxford(2013.01-2016.01). XY, MLJ and SGR acknowledge support from the EPSRC via the programme grant "Materials for Fusion and Fission Power", EP/H018921/1. NR 72 TC 6 Z9 6 U1 11 U2 29 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD JUN 15 PY 2016 VL 112 BP 105 EP 120 DI 10.1016/j.actamat.2016.03.051 PG 16 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA DN8KA UT WOS:000377326400011 ER PT J AU Khafizov, M Pakarinen, J He, L Henderson, HB Manuel, MV Nelson, AT Jaques, BJ Butt, DP Hurley, DH AF Khafizov, M. Pakarinen, J. He, L. Henderson, H. B. Manuel, M. V. Nelson, A. T. Jaques, B. J. Butt, D. P. Hurley, D. H. TI Subsurface imaging of grain microstructure using picosecond ultrasonics SO ACTA MATERIALIA LA English DT Article DE Picosecond ultrasonics; Grain orientation; Boundary characterization ID FOCUSED ION-BEAM; THERMAL-CONDUCTIVITY; URANIUM-DIOXIDE; NANOCRYSTALLINE CERAMICS; OPTICAL-PROPERTIES; THIN-FILMS; BURN-UP; BOUNDARY; UO2; SEGREGATION AB We report on imaging subsurface grain microstructure using picosecond ultrasonics. This approach relies on elastic anisotropy of crystalline materials where ultrasonic velocity depends on propagation direction relative to the crystal axes. Picosecond duration ultrasonic pulses are generated and detected using ultrashort light pulses. In materials that are transparent or semitransparent to the probe wavelength, the probe monitors gigahertz frequency Brillouin oscillations. The frequency of these oscillations is related to the ultrasonic velocity and the optical index of refraction. Ultrasonic waves propagating across a grain boundary experience a change in velocity due to a change in crystallographic orientation relative to the ultrasonic propagation direction. This change in velocity is manifested as a change in the Brillouin oscillation frequency. Using the ultrasonic propagation velocity, the depth of the interface can be determined from the location in time of the transition in oscillation frequency. A subsurface image of the grain boundary is obtained by scanning the beam along the surface. We demonstrate this subsurface imaging capability using a polycrystalline UO2 sample. Cross section liftout analysis of the grain boundary using electron microscopy was used to verify our imaging results. (C) 2016 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Khafizov, M.] Ohio State Univ, Mech & Aerosp Engn, Columbus, OH 43210 USA. [Pakarinen, J.] Belgian Nucl Res Ctr SCK CEN, Boeretang 200, B-2400 Mol, Belgium. [He, L.; Hurley, D. H.] Idaho Natl Lab, Idaho Falls, ID USA. [Henderson, H. B.; Manuel, M. V.] Univ Florida, Mat Sci & Engn, Gainesville, FL 32611 USA. [Nelson, A. T.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. [Jaques, B. J.; Butt, D. P.] Boise State Univ, Mat Sci & Engn, Boise, ID 83725 USA. [Butt, D. P.] Ctr Adv Energy Studies, Idaho Falls, ID 83401 USA. RP Khafizov, M (reprint author), Ohio State Univ, Mech & Aerosp Engn, Columbus, OH 43210 USA.; Hurley, DH (reprint author), Idaho Natl Lab, Idaho Falls, ID USA. EM Khafizov.1@osu.edu; david.hurley@inl.gov RI Khafizov, Marat/B-3744-2012; OI Khafizov, Marat/0000-0001-8171-3528; He, Lingfeng/0000-0003-2763-1462; Nelson, Andrew/0000-0002-4071-3502; Jaques, Brian/0000-0002-5324-555X FU Center for Materials Science of Nuclear Fuel, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [FWP 1356]; U.S. Department of Energy, Office of Nuclear Energy under DOE Idaho Operations Office [DE-AC07-051D14517] FX This material is based upon work supported as part of the Center for Materials Science of Nuclear Fuel, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number FWP 1356. The authors would also like to acknowledge the use of the FIB and EBSD instrumentation at the Center for Advanced Energy Studies which is supported by the U.S. Department of Energy, Office of Nuclear Energy under DOE Idaho Operations Office Contract DE-AC07-051D14517. NR 42 TC 0 Z9 0 U1 11 U2 27 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD JUN 15 PY 2016 VL 112 BP 209 EP 215 DI 10.1016/j.actamat.2016.04.003 PG 7 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA DN8KA UT WOS:000377326400020 ER PT J AU Phan, TQ Levine, LE Lee, IF Xu, RQ Tischler, JZ Huang, Y Langdon, TG Kassner, ME AF Phan, Thien Q. Levine, Lyle E. Lee, I-Fang Xu, Ruqing Tischler, Jonathan Z. Huang, Yi Langdon, Terence G. Kassner, Michael E. TI Synchrotron X-ray microbeam diffraction measurements of full elastic long range internal strain and stress tensors in commercial-purity aluminum processed by multiple passes of equal-channel angular pressing. SO ACTA MATERIALIA LA English DT Article DE Synchrotron X-ray; Diffraction; Full strain tensor; Severe plastic deformation; Aluminum ID MICROSTRUCTURAL EVOLUTION; GRAINED ALUMINUM; COPPER; ECAP; DEFORMATION; REFINEMENT; AL AB Synchrotron X-ray microbeam diffraction was used to measure the full elastic long range internal strain and stress tensors of low dislocation density regions within the submicrometer grain/subgrain structure of equal -channel angular pressed (ECAP) aluminum alloy AA1050 after 1, 2, and 8 passes using route Bc. This is the first time that full tensors were measured in plastically deformed metals at this length scale. The maximum (most tensile or least compressive) principal elastic strain directions for the unloaded 1 pass sample for the grain/subgrain interiors align well with the pressing direction, and are more random for the 2 and 8 pass samples. The measurements reported here indicate that the local stresses and strains become increasingly isotropic (homogenized) with increasing ECAP passes using route B-C. The average maximum (in magnitude) LRISs are -0.43 as for 1 pass, -0.44 sigma(a) for 2 pass, and 0.14 sigma(a) for the 8 pass sample. These LRISs are larger than those reported previously because those earlier measurements were unable to measure the full stress tensor. Significantly, the measured stresses are inconsistent with the two-component composite model. Published by Elsevier Ltd on behalf of Acta Materialia Inc. C1 [Phan, Thien Q.] Univ So Calif, Dept Aerosp & Mech Engn, Los Angeles, CA 90089 USA. [Lee, I-Fang; Langdon, Terence G.; Kassner, Michael E.] Univ So Calif, Dept Chem Engn & Mat Sci, Los Angeles, CA 90089 USA. [Phan, Thien Q.; Levine, Lyle E.] NIST, Mat Sci & Engn Div, Gaithersburg, MD 20899 USA. [Xu, Ruqing; Tischler, Jonathan Z.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Huang, Yi; Langdon, Terence G.] Univ Southampton, Mat Res Grp, Fac Engn & Environm, Southampton SO17 1BJ, Hants, England. RP Phan, TQ (reprint author), NIST, Mat Sci & Engn Div, Gaithersburg, MD 20899 USA. EM thien.phan@nist.gov RI Huang, Yi/E-9008-2012; Langdon, Terence/B-1487-2008 OI Huang, Yi/0000-0001-9259-8123; FU National Science Foundation [DMR-1401194]; DOE Office of Science [DE-AC02-06CH11357]; European Research Council under ERC [267464-SPDMETALS] FX Research at the University of Southern California was supported the National Science Foundation through DMR-1401194, this research used resources of the Advanced Photon Source (beamlines 11-BM and 34-ID-E), a U.S. Department of Energy Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357, and research at the University of Southampton was supported by the European Research Council under ERC Grant Agreement No. 267464-SPDMETALS. NR 26 TC 0 Z9 0 U1 7 U2 9 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD JUN 15 PY 2016 VL 112 BP 231 EP 241 DI 10.1016/j.actamat.2016.04.035 PG 11 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA DN8KA UT WOS:000377326400023 ER PT J AU Raghavan, N Dehoff, R Pannala, S Simunovic, S Kirka, M Turner, J Carlson, N Babu, SS AF Raghavan, Narendran Dehoff, Ryan Pannala, Sreekanth Simunovic, Srdjan Kirka, Michael Turner, John Carlson, Neil Babu, Sudarsanam S. TI Numerical modeling of heat-transfer and the influence of process parameters on tailoring the grain morphology of IN718 in electron beam additive manufacturing SO ACTA MATERIALIA LA English DT Article DE Additive manufacturing; Nickel-base superalloy; Arcam; Microstructure control; Numerical modeling ID INCONEL 718; FLUID-FLOW; LASER; MICROSTRUCTURE; SUPERALLOYS; GROWTH AB The fabrication of 3-D parts from CAD models by additive manufacturing (AM) is a disruptive technology that is transforming the metal manufacturing industry. The correlation between solidification microstructure and mechanical properties has been well understood in the casting and welding processes over the years. This paper focuses on extending these principles to additive manufacturing to understand the transient phenomena of repeated melting and solidification during electron beam powder melting process to achieve site-specific microstructure control within a fabricated component. In this paper, we have developed a novel melt scan strategy for electron beam melting of nickel-base superalloy (Inconel 718) and also analyzed 3-D heat transfer conditions using a parallel numerical solidification code (Truchas) developed at Los Alamos National Laboratory. The spatial and temporal variations of temperature gradient (G) and growth velocity (R) at the liquid-solid interface of the melt pool were calculated as a function of electron beam parameters. By manipulating the relative number of voxels that lie in the columnar or equiaxed region, the crystallographic texture of the components can be controlled to an extent. The analysis of the parameters provided optimum processing conditions that will result in columnar to equiaxed transition (CET) during the solidification. The results from the numerical simulations were validated by experimental processing and characterization thereby proving the potential of additive manufacturing process to achieve site-specific crystallographic texture control within a fabricated component. (C) 2016 Acta Materialia Inc. Published by Elsevier Ltd. All rights reserved. C1 [Raghavan, Narendran] Univ Tennessee, Bredesen Ctr Interdisciplinary Res & Grad Educ, Knoxville, TN 37996 USA. [Dehoff, Ryan; Kirka, Michael; Babu, Sudarsanam S.] Oak Ridge Natl Lab, Mfg Demonstrat Facil, Knoxville, TN 37932 USA. [Dehoff, Ryan; Kirka, Michael] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Pannala, Sreekanth; Simunovic, Srdjan; Turner, John] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37932 USA. [Carlson, Neil] Los Alamos Natl Lab, Computat Phys & Methods, POB 1663,MS D413, Los Alamos, NM 87545 USA. [Babu, Sudarsanam S.] Univ Tennessee, Dept Mech Aerosp & Biomed Engn, Knoxville, TN 37996 USA. RP Raghavan, N (reprint author), Univ Tennessee, 407 Dougherty Engn Bldg, Knoxville, TN 37996 USA. EM naren.ragav@gmail.com RI Dehoff, Ryan/I-6735-2016; OI Dehoff, Ryan/0000-0001-9456-9633; Raghavan, Narendran/0000-0002-6964-5718; Turner, John/0000-0003-2521-4091 FU U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Advanced Manufacturing Office [DE- AC05-00OR22725]; UT-Battelle, LLC; Laboratory Directed Research and Development Program of Oak Ridge National Laboratory; National Nuclear Security Administration of the US Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396]; DOE Advanced Simulation and Computing (ASC) program FX Research was sponsored by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Advanced Manufacturing Office, under contract DE- AC05-00OR22725 with UT-Battelle, LLC. Research was also sponsored by the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory, managed by UT-Battelle, LLC. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. This work was performed, in part, under the auspices of the National Nuclear Security Administration of the US Department of Energy at Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396 and supported by the DOE Advanced Simulation and Computing (ASC) program. NR 38 TC 3 Z9 3 U1 41 U2 96 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD JUN 15 PY 2016 VL 112 BP 303 EP 314 DI 10.1016/j.actamat.2016.03.063 PG 12 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA DN8KA UT WOS:000377326400029 ER PT J AU Song, M Sun, C Fan, Z Chen, Y Zhu, R Yu, KY Hartwig, KT Wang, H Zhang, X AF Song, M. Sun, C. Fan, Z. Chen, Y. Zhu, R. Yu, K. Y. Hartwig, K. T. Wang, H. Zhang, X. TI A roadmap for tailoring the strength and ductility of ferritic/martensitic T91 steel via thermo-mechanical treatment SO ACTA MATERIALIA LA English DT Article DE T91 steel (9Cr-1Mo steel or grade 91); ECAE or ECAP; Thermo-mechanical treatment (TMT); Mechanical properties; Microstructure ID SEVERE PLASTIC-DEFORMATION; AUSTENITIC FE-14CR-16NI ALLOY; CHANNEL ANGULAR EXTRUSION; MODIFIED 9CR-1MO STEEL; MECHANICAL-PROPERTIES; LATH MARTENSITE; GRAIN-SIZE; LOW-CARBON; FE-NI; VARIANT SELECTION AB Ferritic/martensitic (F/M) steels with high strength and excellent ductility are important candidate materials for the life extension of the current nuclear reactors and the design of next generation nuclear reactors. Recent studies show that equal channel angular extrusion (ECAE) was able to improve mechanical strength of ferritic T91 steels moderately. Here, we examine several strategies to further enhance the mechanical strength of T91 while maintaining its ductility. Certain thermo-mechanical treatment (TMT) processes enabled by combinations of ECAE, water quench, and tempering may lead to "ductile martensite" with exceptionally high strength in T91 steel. The evolution of microstructures and mechanical properties of T91 steel were investigated in detail, and transition carbides were identified in water quenched T91 steel. This study provides guidelines for tailoring the microstructure and mechanical properties of T91 steel via ECAE enabled TMT for an improved combination of strength and ductility. Published by Elsevier Ltd on behalf of Acta Materialia Inc. C1 [Song, M.; Chen, Y.; Hartwig, K. T.; Zhang, X.] Texas A&M Univ, Dept Mat Sci & Engn, College Stn, TX 77843 USA. [Sun, C.] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. [Fan, Z.; Zhu, R.; Hartwig, K. T.; Zhang, X.] Texas A&M Univ, Dept Mech Engn, College Stn, TX 77843 USA. [Yu, K. Y.] China Univ Petr, Dept Mat Sci & Engn, Beijing 102249, Peoples R China. [Wang, H.] Texas A&M Univ, Dept Elect Engn, College Stn, TX 77843 USA. [Wang, H.; Zhang, X.] Purdue Univ, Sch Mat Engn, W Lafayette, IN 47907 USA. RP Song, M; Hartwig, KT; Zhang, X (reprint author), Texas A&M Univ, Dept Mat Sci & Engn, College Stn, TX 77843 USA. EM meowsong@umich.edu; thartwig@tamu.edu; xzhang98@purdue.edu RI Chen, Youxing/P-5006-2016 OI Chen, Youxing/0000-0003-1111-4495 FU NSF-DMR-Metallic Materials and Nanostructures Program [1611380]; DOE-NEUP [DE-AC07-05ID14517-00088120]; U.S. Office of Naval Research [N00014-13-10555]; NSF-CMMI [1161978] FX We acknowledge financial support by NSF-DMR-Metallic Materials and Nanostructures Program under grant no. 1611380. M. Song and C. Sun were supported by DOE-NEUP under contract No. DE-AC07-05ID14517-00088120. H. Wang acknowledges the support from the U.S. Office of Naval Research under contract No. N00014-13-10555. Z. Fan is supported by NSF-CMMI under grant No. 1161978. The technical assistance on ECAE processing from Mr. Robert Barber is greatly appreciated. We also acknowledge the microscopy facilities at the Microscopy and Imaging Center (MIC) of Texas A&M University. NR 79 TC 1 Z9 1 U1 9 U2 10 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6454 EI 1873-2453 J9 ACTA MATER JI Acta Mater. PD JUN 15 PY 2016 VL 112 BP 361 EP 377 DI 10.1016/j.actamat.2016.04.031 PG 17 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA DN8KA UT WOS:000377326400034 ER PT J AU Sadovskyy, IA Jia, Y Leroux, M Kwon, J Hu, HF Fang, L Chaparro, C Zhu, SF Welp, U Zuo, JM Zhang, YF Nakasaki, R Selvamanickam, V Crabtree, GW Koshelev, AE Glatz, A Kwok, WK AF Sadovskyy, Ivan A. Jia, Ying Leroux, Maxime Kwon, Jihwan Hu, Hefei Fang, Lei Chaparro, Carlos Zhu, Shaofei Welp, Ulrich Zuo, Jian-Min Zhang, Yifei Nakasaki, Ryusuke Selvamanickam, Venkat Crabtree, George W. Koshelev, Alexei E. Glatz, Andreas Kwok, Wai-Kwong TI Toward Superconducting Critical Current by Design SO ADVANCED MATERIALS LA English DT Article ID HIGH-TEMPERATURE SUPERCONDUCTORS; GINZBURG-LANDAU EQUATION; CRITICAL-CURRENT DENSITY; COLUMNAR DEFECTS; II SUPERCONDUCTORS; HEAVY-IONS; YBA2CU3O7-DELTA; VORTICES; ANISOTROPY AB A new critical-current-by-design paradigm is presented. It aims at predicting the optimal defect landscape in superconductors for targeted applications by elucidating the vortex dynamics responsible for the bulk critical current. To this end, critical current measurements on commercial high-temperature superconductors are combined with large-scale time-dependent Ginzburg-Landau simulations of vortex dynamics. C1 [Sadovskyy, Ivan A.; Jia, Ying; Leroux, Maxime; Fang, Lei; Chaparro, Carlos; Welp, Ulrich; Crabtree, George W.; Koshelev, Alexei E.; Glatz, Andreas; Kwok, Wai-Kwong] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. [Kwon, Jihwan; Zuo, Jian-Min] Univ Illinois, Dept Mat Sci & Engn, 1304 W Green St, Urbana, IL 61801 USA. [Hu, Hefei; Zuo, Jian-Min] Univ Illinois, Mat Res Lab, Urbana, IL 61801 USA. [Fang, Lei] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Zhu, Shaofei] Argonne Natl Lab, Div Phys, 9700 S Cass Ave, Argonne, IL 60439 USA. [Zhang, Yifei; Nakasaki, Ryusuke] SuperPower Corp, Schenectady, NY 12304 USA. [Selvamanickam, Venkat] Univ Houston, Dept Mech Engn, Houston, TX 77204 USA. [Selvamanickam, Venkat] Univ Houston, Texas Ctr Superconduct, Houston, TX 77204 USA. [Crabtree, George W.] Univ Illinois, Dept Phys, Chicago, IL 60607 USA. [Crabtree, George W.] Univ Illinois, Dept Elect Engn, Chicago, IL 60607 USA. [Crabtree, George W.] Univ Illinois, Dept Mech Engn, Chicago, IL 60607 USA. [Glatz, Andreas] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. RP Sadovskyy, IA (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM ivan.sadovsky@gmail.com RI Leroux, Maxime/E-8703-2016; Koshelev, Alexei/K-3971-2013 OI Leroux, Maxime/0000-0001-9778-323X; Koshelev, Alexei/0000-0002-1167-5906 FU Scientific Discovery through Advanced Computing (SciDAC) program - US Department of Energy, Office of Science, Advanced Scientific Computing Research and Basic Energy Science; Center for Emergent Superconductivity, an Energy Frontier Research Center - US Department of Energy, Office of Science, Office of Basic Energy Sciences; US Department of Energy, Office of Nuclear Physics; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX I.A.S., Y.J., and M.L. have contributed equally to this work. The authors thank I. S. Aranson and L. Civale for illuminating discussions. The computational part of our work was performed on the supercomputers Cooley at the LCF at Argonne National Laboratory and GAEA at Northern Illinois University. The computational work was supported by the Scientific Discovery through Advanced Computing (SciDAC) program funded by US Department of Energy, Office of Science, Advanced Scientific Computing Research and Basic Energy Science. The experimental study at ANL was supported by the Center for Emergent Superconductivity, an Energy Frontier Research Center, funded by the US Department of Energy, Office of Science, Office of Basic Energy Sciences. The operation of the ATLAS irradiation facility at ANL was supported by the US Department of Energy, Office of Nuclear Physics. Use of the Center for Nanoscale Materials at ANL was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. This paper is a joint, equally contributed theory-experiment work. NR 47 TC 3 Z9 3 U1 14 U2 43 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD JUN 15 PY 2016 VL 28 IS 23 BP 4593 EP 4600 DI 10.1002/adma.201600602 PG 8 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DO1IO UT WOS:000377531900002 PM 27030115 ER PT J AU Gopal, CB El Gabaly, F McDaniel, AH Chueh, WC AF Gopal, Chirranjeevi Balaji El Gabaly, Farid McDaniel, Anthony H. Chueh, William C. TI Origin and Tunability of Unusually Large Surface Capacitance in Doped Cerium Oxide Studied by Ambient-Pressure X-Ray Photoelectron Spectroscopy SO ADVANCED MATERIALS LA English DT Article ID ELECTROCHEMICAL ENERGY-STORAGE; LOW-INDEX SURFACES; CHEMICAL CAPACITANCE; THIN-FILMS; ELECTRONIC-STRUCTURE; OXYGEN-ION; NONSTOICHIOMETRY; SYSTEM; INTERCALATION; CATALYSIS AB The volumetric redox (chemical) capacitance of the surface of CeO2-delta films is quantified in situ to be 100-fold larger than the bulk values under catalytically relevant conditions. Sm addition slightly lowers the surface oxygen nonstoichiometry, but effects a 10-fold enhancement in surface chemical capacitance by mitigating defect interactions, highlighting the importance of differential nonstoichiometry for catalysis. C1 [Gopal, Chirranjeevi Balaji; Chueh, William C.] Stanford Univ, Dept Mat Sci & Engn, 496 Lomita Mall, Stanford, CA 94305 USA. [El Gabaly, Farid; McDaniel, Anthony H.; Chueh, William C.] Sandia Natl Labs, Livermore, CA 94550 USA. [Chueh, William C.] Stanford Inst Mat & Energy Sci, SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. RP Chueh, WC (reprint author), Stanford Univ, Dept Mat Sci & Engn, 496 Lomita Mall, Stanford, CA 94305 USA.; Chueh, WC (reprint author), Sandia Natl Labs, Livermore, CA 94550 USA.; Chueh, WC (reprint author), Stanford Inst Mat & Energy Sci, SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. EM wchueh@stanford.edu FU Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-AC02-76SF00515]; U.S. Department of Energy through the Sandia Laboratory Directed Research and Development program [DE-AC04-94AL85000]; Office of Science, and Office of Basic Energy Sciences, of the US Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering (Contract No. DE-AC02-76SF00515). Additionally, the research at Sandia was supported by the U.S. Department of Energy through the Sandia Laboratory Directed Research and Development program under Contract No. DE-AC04-94AL85000. W.C.C. was also supported by an appointment to the Sandia National Laboratories Truman Fellowship in National Security Science and Engineering. The Advanced Light Source was supported by the Director, Office of Science, and Office of Basic Energy Sciences, of the US Department of Energy under Contract No. DE-AC02-05CH11231. The authors thank Naila Jabeen and Zhi Liu of the Advanced Light Source for their assistance with ambient pressure X-ray photoelectron spectroscopy experiments, and Sossina Haile and the Kavli Nanoscience Institute at Caltech for providing access to the pulsed-laser deposition facility. NR 47 TC 2 Z9 2 U1 14 U2 37 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD JUN 15 PY 2016 VL 28 IS 23 BP 4692 EP 4697 DI 10.1002/adma.201506333 PG 6 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DO1IO UT WOS:000377531900017 PM 27031580 ER PT J AU Gao, K Miao, JS Xiao, LA Deng, WY Kan, YY Liang, TX Wang, C Huang, F Peng, JB Cao, Y Liu, F Russell, TP Wu, HB Peng, XB AF Gao, Ke Miao, Jingsheng Xiao, Liangang Deng, Wanyuan Kan, Yuanyuan Liang, Tianxiang Wang, Cheng Huang, Fei Peng, Junbiao Cao, Yong Liu, Feng Russell, Thomas P. Wu, Hongbin Peng, Xiaobin TI Multi-Length-Scale Morphologies Driven by Mixed Additives in Porphyrin-Based Organic Photovoltaics SO ADVANCED MATERIALS LA English DT Article ID HETEROJUNCTION SOLAR-CELLS; SMALL-MOLECULE; IMPROVED EFFICIENCY; ENERGY-LOSSES; POLYMER; RECOMBINATION; ANGLE; UNIT AB A new category of deep-absorbing small molecules is developed. Optimized devices driven by mixed additives show a remarkable short-circuit current of approximate to 20 mA cm(-2) and a highest power conversion efficiency of 9.06%. A multi-length-scale morphology is formed, which is fully characterized by resonant soft Xray scattering, high-angle annular dark film image transmission electron microscopy, etc. C1 [Gao, Ke; Miao, Jingsheng; Xiao, Liangang; Deng, Wanyuan; Kan, Yuanyuan; Liang, Tianxiang; Huang, Fei; Peng, Junbiao; Cao, Yong; Wu, Hongbin; Peng, Xiaobin] S China Univ Technol, State Key Lab Luminescent Mat & Devices, Inst Polymer Optoelect Mat & Devices, 381 Wushan Rd, Guangzhou 510640, Guangdong, Peoples R China. [Wang, Cheng] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Liu, Feng; Russell, Thomas P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Russell, Thomas P.] Univ Massachusetts, Polymer Sci & Engn Dept, Amherst, MA 01003 USA. RP Wu, HB; Peng, XB (reprint author), S China Univ Technol, State Key Lab Luminescent Mat & Devices, Inst Polymer Optoelect Mat & Devices, 381 Wushan Rd, Guangzhou 510640, Guangdong, Peoples R China.; Liu, F; Russell, TP (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.; Russell, TP (reprint author), Univ Massachusetts, Polymer Sci & Engn Dept, Amherst, MA 01003 USA. EM iamfengliu@gmail.com; russell@mail.pse.umass.edu; hbwu@scut.edu.cn; chxbpeng@scut.edu.cn RI Gao, Ke/B-3412-2017; Wang, Cheng/A-9815-2014; Liu, Feng/J-4361-2014 OI Liu, Feng/0000-0002-5572-8512 FU International Science & Technology Cooperation Program of China [2013DFG52740, 2010DFA52150]; Ministry of Science and Technology [2014CB643500]; National Natural Science Foundation of China [51473053, 51073060]; U.S. Office of Naval Research [N00014-15-1-2244]; DOE; Office of Science; Office of Basic Energy Sciences FX K.G. and J.M. contributed equally to this work. This work was financially supported by the grants from the International Science & Technology Cooperation Program of China (2013DFG52740, 2010DFA52150), the Ministry of Science and Technology (2014CB643500), and the National Natural Science Foundation of China (51473053, 51073060). F.L. and T.P.R. were supported by the U.S. Office of Naval Research under contract N00014-15-1-2244. Portions of this research were carried out at beamline 7.3.3 and 11.0.1.2 at the Advanced Light Source, Molecular Foundry, and the National Center for Electron Micoscopy, Lawrence Berkeley National Laboratory, which was supported by the DOE, the Office of Science, and the Office of Basic Energy Sciences. NR 35 TC 14 Z9 14 U1 32 U2 81 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD JUN 15 PY 2016 VL 28 IS 23 BP 4727 EP 4733 DI 10.1002/adma.201505645 PG 7 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DO1IO UT WOS:000377531900022 PM 27062394 ER PT J AU Lerma-Ortiz, C Jeffryes, JG Cooper, AJL Niehaus, TD Thamm, AMK Frelin, O Aunins, T Fiehn, O de Crecy-Lagard, V Henry, CS Hanson, AD AF Lerma-Ortiz, Claudia Jeffryes, James G. Cooper, Arthur J. L. Niehaus, Thomas D. Thamm, Antje M. K. Frelin, Oceane Aunins, Thomas Fiehn, Oliver de Crecy-Lagard, Valerie Henry, Christopher S. Hanson, Andrew D. TI 'Nothing of chemistry disappears in biology': the Top 30 damage-prone endogenous metabolites SO BIOCHEMICAL SOCIETY TRANSACTIONS LA English DT Review DE computational biochemistry; metabolite damage; metabolome; side-product; side reaction; spontaneous chemistry ID GENOME-SCALE RECONSTRUCTION; ESCHERICHIA-COLI; CARBAMOYL-PHOSPHATE; UNTARGETED METABOLOMICS; RIBOFLAVIN BIOSYNTHESIS; ENZYME PROMISCUITY; BACILLUS-SUBTILIS; MECHANISM; PATHWAYS; MODELS AB Many common metabolites are intrinsically unstable and reactive, and hence prone to chemical (i.e. nonenzymatic) damage in vivo. Although this fact is widely recognized, the purely chemical side-reactions of metabolic intermediates can be surprisingly hard to track down in the literature and are often treated in an unprioritized case-by-case way. Moreover, spontaneous chemical side-reactions tend to be overshadowed today by side-reactions mediated by promiscuous ('sloppy') enzymes even though chemical damage to metabolites may be even more prevalent than damage from enzyme sloppiness, has similar outcomes, and is held in check by similar biochemical repair or pre-emption mechanisms. To address these limitations and imbalances, here we draw together and systematically integrate information from the (bio) chemical literature, from cheminformatics, and from genome-scale metabolic models to objectively define a 'Top 30' list of damage-prone metabolites. A foundational part of this process was to derive general reaction rules for the damage chemistries involved. The criteria for a 'Top 30' metabolite included predicted chemical reactivity, essentiality, and occurrence in diverse organisms. We also explain how the damage chemistry reaction rules ('operators') are implemented in the Chemical-Damage-MINE (CD-MINE) database (minedatabase.mcs.anl.gov/#/top30) to provide a predictive tool for many additional potential metabolite damage products. Lastly, we illustrate how defining a 'Top 30' list can drive genomics-enabled discovery of the enzymes of previously unrecognized damage-control systems, and how applying chemical damage reaction rules can help identify previously unknown peaks in metabolomics profiles. C1 [Lerma-Ortiz, Claudia; de Crecy-Lagard, Valerie] Univ Florida, Microbiol & Cell Sci Dept, Gainesville, FL 32611 USA. [Jeffryes, James G.; Aunins, Thomas; Henry, Christopher S.] Northwestern Univ, Dept Chem & Biol Engn, Evanston, IL 60208 USA. [Jeffryes, James G.; Henry, Christopher S.] Argonne Natl Lab, Math & Comp Sci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Cooper, Arthur J. L.] New York Med Coll, Dept Biochem & Mol Biol, Valhalla, NY 10595 USA. [Niehaus, Thomas D.; Thamm, Antje M. K.; Frelin, Oceane; Hanson, Andrew D.] Univ Florida, Dept Hort Sci, Gainesville, FL 32611 USA. [Fiehn, Oliver] Univ Calif Davis, Genome Ctr, Davis, CA 95616 USA. RP Henry, CS (reprint author), Northwestern Univ, Dept Chem & Biol Engn, Evanston, IL 60208 USA.; Henry, CS (reprint author), Argonne Natl Lab, Math & Comp Sci Div, 9700 S Cass Ave, Argonne, IL 60439 USA.; Hanson, AD (reprint author), Univ Florida, Dept Hort Sci, Gainesville, FL 32611 USA. EM chenry@ci.uchicago.edu; adha@ufl.edu FU US National Science Foundation [MCB-1153413, MCB-1153357, MCB-1153491] FX The work was supported by the US National Science Foundation [grant numbers MCB-1153413 (to A.D.H.), MCB-1153357 (to C.S.H.) and MCB-1153491 (to O.F.)]. NR 60 TC 3 Z9 3 U1 12 U2 24 PU PORTLAND PRESS LTD PI LONDON PA CHARLES DARWIN HOUSE, 12 ROGER STREET, LONDON WC1N 2JU, ENGLAND SN 0300-5127 EI 1470-8752 J9 BIOCHEM SOC T JI Biochem. Soc. Trans. PD JUN 15 PY 2016 VL 44 BP 961 EP 971 DI 10.1042/BST20160073 PN 3 PG 11 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA DO1EN UT WOS:000377521400044 PM 27284066 ER PT J AU Zheng, ZT Zhu, WQ Chen, GS Jiang, N Fan, DQ Zhang, DH AF Zheng, Zhoutao Zhu, Wenquan Chen, Guangsheng Jiang, Nan Fan, Deqin Zhang, Donghai TI Continuous but diverse advancement of spring-summer phenology in response to climate warming across the Qinghai-Tibetan Plateau SO AGRICULTURAL AND FOREST METEOROLOGY LA English DT Article DE Climate change; Spring-summer phenology; Phenology shift; Climatic sensitivity; Qinghai-Tibetan Plateau ID VEGETATION GREEN-UP; LAST DECADE; NO EVIDENCE; WINTER; CHINA; METAANALYSIS; TREND; MODEL; DATES AB The Qinghai-Tibetan Plateau (QTP) is more vulnerable and sensitive to climate change than many other regions worldwide because of its high altitude, permafrost geography, and harsh physical environment. As a sensitive bio-indicator of climate change, plant phenology shift in this region has been intensively studied during the recent decades, primarily based on satellite-retrieved data. However, great controversy still exists regarding the change in direction and magnitudes of spring-summer phenology. Based on a large number (11,000+ records) of long-term and continuous ground observational data for various plant species, our study intended to more comprehensively assess the changing trends of spring-summer phenology and their relationships with climatic change across the QTP. The results indicated a continuous advancement (-2.69 days decade(-1)) in spring-summer phenology from 1981 to 2011, with an even more rapid advancement during 2000-2011 (-3.13 days decade-1), which provided new field evidence for continuous advancement in spring-summer phenology across the QTP. However, diverse advancing rates in spring-summer phenology were observed for different vegetation types, thermal conditions, and seasons. The advancing trends matched well with the difference in sensitivity of spring-summer phenology to increasing temperature, implying that the sensitivity of phenology to temperature was one of the major factors influencing spring-summer phenology shifts. Besides, increased precipitation could advance the spring-summer phenology. The response of spring-summer phenology to temperature tended to be stronger from east to west across all species, while the response to precipitation showed no consistent spatial pattern. (C) 2016 Elsevier B.V. All rights reserved. C1 [Zheng, Zhoutao; Zhu, Wenquan; Jiang, Nan; Fan, Deqin; Zhang, Donghai] Beijing Normal Univ, State Key Lab Earth Surface Proc & Resource Ecol, Beijing 100875, Peoples R China. [Zheng, Zhoutao; Zhu, Wenquan; Jiang, Nan; Fan, Deqin; Zhang, Donghai] JCGCS, Beijing 100875, Peoples R China. [Zheng, Zhoutao; Zhu, Wenquan; Jiang, Nan; Fan, Deqin; Zhang, Donghai] Beijing Normal Univ, Coll Resources Sci & Technol, Beijing 100875, Peoples R China. [Chen, Guangsheng] Oak Ridge Natl Lab, Div Environm Sci, POB 2008, Oak Ridge, TN 37831 USA. RP Zhu, WQ (reprint author), Beijing Normal Univ, Coll Resources Sci & Technol, Beijing 100875, Peoples R China. EM zhuwq75@bnu.edu.cn FU National Natural Science Foundation of China [41371389]; State Key Laboratory of Earth Surface Processes and Resource Ecology [2013-ZY-14] FX This work was supported by the National Natural Science Foundation of China (No. 41371389) and the State Key Laboratory of Earth Surface Processes and Resource Ecology (No. 2013-ZY-14). NR 43 TC 0 Z9 0 U1 7 U2 23 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-1923 EI 1873-2240 J9 AGR FOREST METEOROL JI Agric. For. Meteorol. PD JUN 15 PY 2016 VL 223 BP 194 EP 202 DI 10.1016/j.agrformet.2016.04.012 PG 9 WC Agronomy; Forestry; Meteorology & Atmospheric Sciences SC Agriculture; Forestry; Meteorology & Atmospheric Sciences GA DN1OJ UT WOS:000376835000017 ER PT J AU Luo, HX Yan, K Pletikosic, I Xie, WW Phelan, BF Valla, T Cava, RJ AF Luo, Huixia Yan, Kai Pletikosic, Ivo's Xie, Weiwei Phelan, Brendan F. Valla, Tonica Cava, Robert J. TI Superconductivity in a Misfit Phase That Combines the Topological Crystalline Insulator Pb1-xSnxSe with the CDW-Bearing Transition Metal Dichalcogenide TiSe2 SO JOURNAL OF THE PHYSICAL SOCIETY OF JAPAN LA English DT Article ID NB-SE SYSTEM; LAYER COMPOUNDS; TERNARY SELENIDES; COMPOSITE; INTERCALATION; (PBS)1.12VS2; TRANSPORT AB We report the characterization of the misfit compound (Pb1-xSnxSe2)(1.16)(TiSe2)(2) for 0 <= x <= 0.6, in which a [100] rocksalt-structure bilayer of Pb1-xSnxSe, which is a topological crystalline insulator in bulk form, alternates with a double layer of the normally non-superconducting transition metal dichalcogenide TiSe2. The x dependence of T-c displays a weak dome-like shape with a maximum T-c of 4.5 K at x = 0.2; there is only a subtle change in T-c at the composition where the trivial to topological transition occurs in bulk Pb1-xSnxSe. We present the characterization of the superconductor at x = 0.4, for which the bulk Pb1-xSnxSe phase is in the topological crystalline insulator regime. For this material, the Sommerfeld parameter gamma = 11.06 mJ mol(-1)K(-2), the Debye temperature Theta(D) = 161 K, the normalized specific heat jump value Delta C/gamma T-c = 1.38 and the electron-phonon constant value lambda(ep) = 0.72, suggesting that (Pb0.6Sn0.4Se)(1.16)(TiSe2)(2) is a BCS-type weak coupling superconductor. This material may be of interest for probing the interaction of superconductivity with the surface states of a topological crystalline insulator. C1 [Luo, Huixia; Xie, Weiwei; Phelan, Brendan F.; Cava, Robert J.] Princeton Univ, Dept Chem, Princeton, NJ 08544 USA. [Yan, Kai] Brown Univ, Sch Engn, Providence, RI 02912 USA. [Pletikosic, Ivo's; Valla, Tonica] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Pletikosic, Ivo's] Princeton Univ, Dept Phys, Princeton, NJ 08544 USA. RP Luo, HX; Cava, RJ (reprint author), Princeton Univ, Dept Chem, Princeton, NJ 08544 USA. EM huixial@princeton.edu; rcava@princeton.edu RI Luo, huixia/A-7544-2014; Yan, Kai/H-7191-2016; Pletikosic, Ivo/A-5683-2010; Luo, Huixia/D-8467-2017 OI Luo, huixia/0000-0003-0999-6441; Pletikosic, Ivo/0000-0003-4697-8912; Luo, Huixia/0000-0003-2703-5660 FU Department of Energy, division of basic energy sciences [DE-FG02-98ER45706]; ARO MURI [W911NF-12-0461] FX The materials synthesis and physical property characterization of this superconductor were supported by the Department of Energy, division of basic energy sciences, Grant DE-FG02-98ER45706. The ARPES work was supported by the ARO MURI on topological insulators grant W911NF-12-0461. The authors acknowledge discussions with Ali Yazdani. NR 30 TC 0 Z9 0 U1 8 U2 31 PU PHYSICAL SOC JAPAN PI TOKYO PA YUSHIMA URBAN BUILDING 5F, 2-31-22 YUSHIMA, BUNKYO-KU, TOKYO, 113-0034, JAPAN SN 0031-9015 J9 J PHYS SOC JPN JI J. Phys. Soc. Jpn. PD JUN 15 PY 2016 VL 85 IS 6 AR 064705 DI 10.7566/JPSJ.85.064705 PG 5 WC Physics, Multidisciplinary SC Physics GA DN0PB UT WOS:000376764700023 ER PT J AU Watanabe, H Vishwanath, A AF Watanabe, Haruki Vishwanath, Ashvin TI Electric Field-Induced Skyrmion Crystals via Charged Monopoles in Insulating Helimagets SO JOURNAL OF THE PHYSICAL SOCIETY OF JAPAN LA English DT Article ID MAGNETIC MONOPOLES; LATTICE AB Electrons propagating in a magnetically ordered medium experience an additional gauge field associated with the Berry phase of their spin following the local magnetic texture. In contrast to the usual electromagnetic field, this gauge field admits monopole excitations, corresponding to hedgehog defects of the magnetic order. In an insulator, these hedgehogs carry a well-defined electric charge allowing for them to be controlled by electric fields. One particularly robust mechanism that contributes to the charge is the orbital magnetoelectric effect, captured by a theta angle, which leads to a charge of e theta/2 pi on hedgehogs. This is a direct consequence of the Witten effect for magnetic monopoles in a theta medium. A physical consequence is that external electric fields can induce skyrmion crystal phases in insulating helimagnets. C1 [Watanabe, Haruki; Vishwanath, Ashvin] Univ Tokyo, Dept Appl Phys, Bunkyo Ku, Tokyo 1138656, Japan. [Vishwanath, Ashvin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Watanabe, H (reprint author), Univ Tokyo, Dept Appl Phys, Bunkyo Ku, Tokyo 1138656, Japan. EM hwatanabe@berkeley.edu FU ARO MURI [W911-NF-12-1-0961] FX We thank Oleg Tchernyshyov for useful comments. This research was supported by the ARO MURI on topological insulators grant W911-NF-12-1-0961. NR 22 TC 2 Z9 2 U1 5 U2 18 PU PHYSICAL SOC JAPAN PI TOKYO PA YUSHIMA URBAN BUILDING 5F, 2-31-22 YUSHIMA, BUNKYO-KU, TOKYO, 113-0034, JAPAN SN 0031-9015 J9 J PHYS SOC JPN JI J. Phys. Soc. Jpn. PD JUN 15 PY 2016 VL 85 IS 6 AR 064707 DI 10.7566/JPSJ.85.064707 PG 5 WC Physics, Multidisciplinary SC Physics GA DN0PB UT WOS:000376764700025 ER PT J AU Ghimire, NJ Botana, AS Phelan, D Zheng, H Mitchell, JF AF Ghimire, N. J. Botana, A. S. Phelan, D. Zheng, H. Mitchell, J. F. TI Magnetotransport of single crystalline YSb SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE topologial insulator; Weyl semimetal; Dirac semimetal; surface states ID WEYL FERMION SEMIMETAL; TOPOLOGICAL INSULATORS; GIANT MAGNETORESISTANCE; ULTRAHIGH MOBILITY; METAL; ARCS; TAAS AB We report magnetic field dependent transport measurements on a single crystal of cubic YSb together with first principles calculations of its electronic structure. The transverse magnetoresistance does not saturate up to 9 T and attains a value of 75 000% at 1.8 K. The Hall coefficient is electron-like at high temperature, changes sign to hole-like between 110 and 50 K, and again becomes electron-like below 50 K. First principles calculations show that YSb is a compensated semimetal with a qualitatively similar electronic structure to that of isostructural LaSb and LaBi, but with larger Fermi surface volume. The measured electron carrier density and Hall mobility calculated at 1.8 K, based on a single band approximation, are 6.5x10(20) cm(-3) and 6.2x10(4) cm(2) Vs(-1), respectively. These values are comparable with those reported for LaBi and LaSb. Like LaBi and LaSb, YSb undergoes a magnetic field-induced metal-insulator-like transition below a characteristic temperature T-m, with resistivity saturation below 13 K. Thickness dependent electrical resistance measurements show a deviation of the resistance behavior from that expected for a normal metal; however, they do not unambiguously establish surface conduction as the mechanism for the resistivity plateau. C1 [Ghimire, N. J.; Botana, A. S.; Phelan, D.; Zheng, H.; Mitchell, J. F.] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Ghimire, NJ (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM nghimire@anl.gov FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Science and Engineering Division FX This work was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Science and Engineering Division. The authors thank D Y Chung for his help during the crystal growth. NR 38 TC 4 Z9 4 U1 23 U2 58 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD JUN 15 PY 2016 VL 28 IS 23 AR 235601 DI 10.1088/0953-8984/28/23/235601 PG 7 WC Physics, Condensed Matter SC Physics GA DM5SP UT WOS:000376410700008 PM 27160492 ER PT J AU Neupane, M Hosen, MM Belopolski, I Wakeham, N Dimitri, K Dhakal, N Zhu, JX Hasan, MZ Bauer, ED Ronning, F AF Neupane, Madhab Hosen, M. Mofazzel Belopolski, Ilya Wakeham, Nicholas Dimitri, Klauss Dhakal, Nagendra Zhu, Jian-Xin Hasan, M. Zahid Bauer, Eric D. Ronning, Filip TI Observation of Dirac-like semi-metallic phase in NdSb SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE topological; semi-metal; Dirac; ARPES; NdSb; rare earth monopnictide ID WEYL FERMION SEMIMETAL; TOPOLOGICAL INSULATORS; ELECTRONIC-STRUCTURE; ULTRAHIGH MOBILITY; MAGNETORESISTANCE; SURFACE; CD3AS2; ARCS AB The search of new topological phases of matter is one of the new directions in condensed matter physics. Recent experimental realizations of Dirac semimetal phases pave the way to look for other exotic phases of matter in real materials. Here we present a systematic angle-resolved photoemission spectroscopy (ARPES) study of NdSb, a potential candidate for hosting a Dirac semi-metal phase. Our studies reveal two hole-like Fermi surface pockets present at the zone center (Gamma) point as well as two elliptical electron-pockets present in the zone corner (X) point of the Brillouin zone (BZ). Interestingly, Dirac-like linearly dispersive states are observed about the zone corner (X) point in NdSb. Our first-principles calculations agree with the experimentally observed bands at the Gamma point. Moreover, the Dirac-like state observed in NdSb may be a novel correlated state, not yet predicted in calculations. Our study opens a new direction to look for Dirac semi-metal states in other members of the rare earth monopnictide family. C1 [Neupane, Madhab; Hosen, M. Mofazzel; Dimitri, Klauss; Dhakal, Nagendra] Univ Cent Florida, Dept Phys, Orlando, FL 32816 USA. [Belopolski, Ilya; Hasan, M. Zahid] Princeton Univ, Joseph Henry Lab, Princeton, NJ 08544 USA. [Belopolski, Ilya; Hasan, M. Zahid] Princeton Univ, Dept Phys, Princeton, NJ 08544 USA. [Wakeham, Nicholas; Bauer, Eric D.; Ronning, Filip] Los Alamos Natl Lab, Condensed Matter & Magnet Sci Grp, POB 1663, Los Alamos, NM 87545 USA. [Zhu, Jian-Xin] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Neupane, M (reprint author), Univ Cent Florida, Dept Phys, Orlando, FL 32816 USA. EM Madhab.Neupane@ucf.edu OI Ronning, Filip/0000-0002-2679-7957; Bauer, Eric/0000-0003-0017-1937 FU University of Central Florida (UCF); NSF GRFP; Emergent Phenomena in Quantum Systems Initiative of the Gordon and Betty Moore Foundation [GBMF4547]; National Science Foundation, Division of Materials Research [NSF-DMR-1507585, NSF-DMR-1006492]; U.S. Department of Energy, Office of Science; Los Alamos National Laboratory LDRD program FX MN is supported by the start-up fund from University of Central Florida (UCF). IB acknowledges the support of the NSF GRFP. Work at Princeton University is supported by the Emergent Phenomena in Quantum Systems Initiative of the Gordon and Betty Moore Foundation under Grant No. GBMF4547 (M.Z.H.) and by the National Science Foundation, Division of Materials Research, under Grants No. NSF-DMR-1507585 and No. NSF-DMR-1006492. Synthesis and transport measurements of the crystals were performed at Los Alamos National Laboratory under the auspices of the U.S. Department of Energy, Office of Science. Electronic structure calculations were performed with the support of the Los Alamos National Laboratory LDRD program. We thank Plumb Nicholas Clark for beamline assistance at the SLS, PSI. We also thank Sung-Kwan Mo for beamline assistance at the LBNL. MN acknowledges fruitful discussions with T Durakiewicz and A V Balatsky at LANL, and Talat Rahman at UCF. NR 30 TC 2 Z9 2 U1 12 U2 36 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD JUN 15 PY 2016 VL 28 IS 23 AR 23LT02 DI 10.1088/0953-8984/28/23/23LT02 PG 5 WC Physics, Condensed Matter SC Physics GA DM5SP UT WOS:000376410700002 PM 27156499 ER PT J AU Law, KJH Sanz-Alonso, D Shukla, A Stuart, AM AF Law, K. J. H. Sanz-Alonso, D. Shukla, A. Stuart, A. M. TI Filter accuracy for the Lorenz 96 model: Fixed versus adaptive observation operators SO PHYSICA D-NONLINEAR PHENOMENA LA English DT Article DE 3DVAR; Lorenz '96; Filter accuracy; Adaptive observations; Extended Kalman filter ID CONTINUOUS DATA ASSIMILATION; UNSTABLE SUBSPACE; KALMAN FILTER AB In the context of filtering chaotic dynamical systems it is well-known that partial observations, if sufficiently informative, can be used to control the inherent uncertainty due to chaos. The purpose of this paper is to investigate, both theoretically and numerically, conditions on the observations of chaotic systems under which they can be accurately filtered. In particular, we highlight the advantage of adaptive observation operators over fixed ones. The Lorenz '96 model is used to exemplify our findings. We consider discrete-time and continuous-time observations in our theoretical developments. We prove that, for fixed observation operator, the 3DVAR filter can recover the system state within a neighbourhood determined by the size of the observational noise. It is required that a sufficiently large proportion of the state vector is observed, and an explicit form for such sufficient fixed observation operator is given. Numerical experiments, where the data is incorporated by use of the 3DVAR and extended Kalman filters, suggest that less informative fixed operators than given by our theory can still lead to accurate signal reconstruction. Adaptive observation operators are then studied numerically; we show that, for carefully chosen adaptive observation operators, the proportion of the state vector that needs to be observed is drastically smaller than with a fixed observation operator. Indeed, we show that the number of state coordinates that need to be observed may even be significantly smaller than the total number of positive Lyapunov exponents of the underlying system. (C) 2016 Published by Elsevier B.V. C1 [Law, K. J. H.] Oak Ridge Natl Lab, Div Comp Sci & Math, Oak Ridge, TN 37831 USA. [Sanz-Alonso, D.; Shukla, A.; Stuart, A. M.] Univ Warwick, Math Inst, Coventry CV4 7AL, W Midlands, England. RP Shukla, A (reprint author), Univ Warwick, Math Inst, Coventry CV4 7AL, W Midlands, England. EM a.shukla@warwick.ac.uk OI Law, Kody/0000-0003-3133-2537 FU EPSRC-MASDOC graduate training scheme; EPSRC; ERC; ONR; King Abdullah University of Science and Technology FX AbS and DSA are supported by the EPSRC-MASDOC graduate training scheme. AMS is supported by EPSRC, ERC and ONR. KJHL is supported by King Abdullah University of Science and Technology, and is a member of the KAUST SRI-UQ Center. NR 20 TC 1 Z9 1 U1 0 U2 4 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-2789 EI 1872-8022 J9 PHYSICA D JI Physica D PD JUN 15 PY 2016 VL 325 BP 1 EP 13 DI 10.1016/j.physd.2015.12.008 PG 13 WC Mathematics, Applied; Physics, Multidisciplinary; Physics, Mathematical SC Mathematics; Physics GA DM9QH UT WOS:000376700300001 ER PT J AU Duanmu, M Whitaker, N Kevrekidis, PG Vainchtein, A Rubin, JE AF Duanmu, M. Whitaker, N. Kevrekidis, P. G. Vainchtein, A. Rubin, J. E. TI Traveling wave wave solutions in a chain of periodically forced coupled nonlinear oscillators SO PHYSICA D-NONLINEAR PHENOMENA LA English DT Article DE Coupled nonlinear oscillators; Discrete model; Traveling waves ID SOLITARY WAVES; FPU LATTICES; DYNAMICS; PHOSPHENES; STABILITY; BREATHERS; INDUCTION; NETWORK; VISION; DNA AB Motivated by earlier studies of artificial perceptions of light called phosphenes, we analyze traveling wave solutions in a chain of periodically forced coupled nonlinear oscillators modeling this phenomenon. We examine the discrete model problem in its co-traveling frame and systematically obtain the corresponding traveling waves in one spatial dimension. Direct numerical simulations as well as linear stability analysis are employed to reveal the parameter regions where the traveling waves are stable, and these waves are, in turn, connected to the standing waves analyzed in earlier work. We also consider a two-dimensional extension of the model and demonstrate the robust evolution and stability of planar fronts. Our simulations also suggest the radial fronts tend to either annihilate or expand and flatten out, depending on the phase value inside and the parameter regime. Finally, we observe that solutions that initially feature two symmetric fronts with bulged centers evolve in qualitative agreement with experimental observations of phosphenes. (C) 2016 Elsevier B.V. All rights reserved. C1 [Duanmu, M.; Whitaker, N.; Kevrekidis, P. G.] Univ Massachusetts, Dept Math & Stat, Amherst, MA 01003 USA. [Kevrekidis, P. G.] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. [Kevrekidis, P. G.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Vainchtein, A.; Rubin, J. E.] Univ Pittsburgh, Dept Math, Pittsburgh, PA 15260 USA. [Rubin, J. E.] Univ Pittsburgh, Ctr Neural Basis Cognit, Pittsburgh, PA 15260 USA. RP Whitaker, N (reprint author), Univ Massachusetts, Dept Math & Stat, Amherst, MA 01003 USA. EM whitaker@math.umass.edu FU US-AFOSR [FA9550-12-1-0332]; ERC under FP7, Marie Curie Actions, People, International Research Staff Exchange Scheme [IRSES-605096]; US Department of Energy; NSF award [DMS-1312508] FX PGK gratefully acknowledges the support of the US-AFOSR under grant FA9550-12-1-0332, and the ERC under FP7, Marie Curie Actions, People, International Research Staff Exchange Scheme (IRSES-605096). Some of PGK's work on the manuscript was done during his one-year residence as an Ulam fellow at the Center for Nonlinear Studies, Los Alamos National Laboratory, supported in part by the US Department of Energy. JER was partially supported by the NSF award DMS-1312508. NR 29 TC 0 Z9 0 U1 3 U2 3 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-2789 EI 1872-8022 J9 PHYSICA D JI Physica D PD JUN 15 PY 2016 VL 325 BP 25 EP 40 DI 10.1016/j.physd.2016.02.001 PG 16 WC Mathematics, Applied; Physics, Multidisciplinary; Physics, Mathematical SC Mathematics; Physics GA DM9QH UT WOS:000376700300003 ER PT J AU Bracco, JN Gooijer, Y Higgins, SR AF Bracco, Jacquelyn N. Gooijer, Yiscka Higgins, Steven R. TI Hydrothermal atomic force microscopy observations of barite step growth rates as a function of the aqueous barium-to-sulfate ratio SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article ID SCANNING PROBE MICROSCOPY; KOSSEL CRYSTAL-GROWTH; CALCITE GROWTH; SOLUTION STOICHIOMETRY; CONSTANT SUPERSATURATION; DISSOLUTION KINETICS; SATURATION STATE; IONIC-STRENGTH; KINK DYNAMICS; SURFACE AB The rate of growth of ionic minerals from solutions with varying aqueous cation: anion ratios may result in significant errors in mineralization rates predicted by commonly-used affinity-based rate equations. To assess the potential influence of solute stoichiometry on barite growth, step velocities on the barite (001) surface have been measured at 108 degrees C using hydrothermal atomic force microscopy (HAFM) at moderate supersaturation and as a function of the aqueous barium: sulfate ratio (r). Barite growth hillocks at r similar to 1 were bounded by < 120 > steps, however at r < 1, kink site densities increased, steps followed a direction vicinal to < 120 >, and the [010] steps developed. At r > 1, steps roughened and rounded as the kink site density increased. Step velocities peaked at r = 1 and decreased roughly symmetrically as a function of r, indicating the attachment rates of barium and sulfate ions are similar under these conditions. We hypothesize that the differences in our observations at high and low r arise from differences in the attachment rate constants for the obtuse and acute < 120 > steps. Based on results at low r, the data suggests the attachment rate constant for barium ions is similar for obtuse and acute steps. Based on results at high r, the data suggests the attachment rate constant for sulfate is greater for obtuse steps than acute steps. Utilizing a step growth model developed by Stack and Grantham (2010) the experimental step velocities as a function of r were readily fit while attempts to fit the data using a model developed by Zhang and Nancollas (1998) were less successful. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Bracco, Jacquelyn N.; Gooijer, Yiscka; Higgins, Steven R.] Wright State Univ, Dept Chem, 3640 Col Glenn Hwy, Dayton, OH 45435 USA. [Gooijer, Yiscka] Hgsk Utrecht, Inst Life Sci & Chem, Utrecht, Netherlands. [Bracco, Jacquelyn N.] Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Higgins, SR (reprint author), Wright State Univ, Dept Chem, 3640 Col Glenn Hwy, Dayton, OH 45435 USA. OI Bracco, Jacquelyn/0000-0002-7096-8856 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division FX This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division. We are grateful to Garrett VanNess for technical assistance, to Andrew Stack for helpful discussions and providing the mineral samples and to two anonymous reviewers for their suggestions for improving the manuscript. NR 48 TC 2 Z9 2 U1 18 U2 24 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 EI 1872-9533 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD JUN 15 PY 2016 VL 183 BP 1 EP 13 DI 10.1016/j.gca.2016.03.009 PG 13 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA DM2HP UT WOS:000376168000001 ER PT J AU Syracuse, EM Maceira, M Prieto, GA Zhang, HJ Ammon, CJ AF Syracuse, Ellen M. Maceira, Monica Prieto, German A. Zhang, Haijiang Ammon, Charles J. TI Multiple plates subducting beneath Colombia, as illuminated by seismicity and velocity from the joint inversion of seismic and gravity data SO EARTH AND PLANETARY SCIENCE LETTERS LA English DT Article DE flat-slab; Bucaramanga nest; slab tear; body wave; surface wave; gravity ID NORTHWESTERN SOUTH-AMERICA; SURFACE-WAVE DISPERSION; NORTHERN ANDES; OCEANIC LITHOSPHERE; FOCAL MECHANISMS; HAYWARD FAULT; UPPER-MANTLE; EARTHQUAKES; TOMOGRAPHY; ZONE AB Subduction beneath the northernmost Andes in Colombia is complex. Based on seismicity distributions, multiple segments of slab appear to be subducting, and arc volcanism ceases north of 5 degrees N. Here, we illuminate the subduction system through hypocentral relocations and Vp and Vs models resulting from the joint inversion of local body wave arrivals, surface wave dispersion measurements, and gravity data. The simultaneous use of multiple data types takes advantage of the differing sensitivities of each data type, resulting in velocity models that have improved resolution at both shallower and deeper depths than would result from traditional travel time tomography alone. The relocated earthquake dataset and velocity model clearly indicate a tear in the Nazca slab at 5 degrees N, corresponding to a 250-km shift in slab seismicity and the termination of arc volcanism. North of this tear, the slab is flat, and it comprises slabs of two sources: the Nazca and Caribbean plates. The Bucaramanga nest, a small region of among the most intense intermediate-depth seismicity globally, is associated with the boundary between these two plates and possibly with a zone of melting or elevated water content, based on reduced Vp and increased Vp/Vs. We also use relocated seismicity to identify two new faults in the South American plate, one related to plate convergence and one highlighted by induced seismicity. (C) 2016 Published by Elsevier B.V. C1 [Syracuse, Ellen M.; Maceira, Monica] Los Alamos Natl Lab, EES 17, POB 1663,MS F665, Los Alamos, NM 87545 USA. [Prieto, German A.] MIT, Dept Earth Atmospher & Planetary Sci, 77 Massachusetts Ave, Cambridge, MA 01239 USA. [Zhang, Haijiang] Univ Sci & Technol China, Sch Earth & Space Sci, Lab Seismol & Phys Earths Interior, 96 Jinzhai Rd, Hefei 230026, Anhui, Peoples R China. [Ammon, Charles J.] Penn State Univ, Dept Geosci, 440 Deike Bldg, University Pk, PA 16802 USA. RP Syracuse, EM (reprint author), Los Alamos Natl Lab, EES 17, POB 1663,MS F665, Los Alamos, NM 87545 USA. EM syracuse@lanl.gov RI Prieto, German/B-8833-2008; OI Prieto, German/0000-0001-8538-7379; Maceira, Monica/0000-0003-1248-2185; Syracuse, Ellen/0000-0002-8145-8480 FU Los Alamos National Laboratory Director's Postdoctoral fellowship [LDRD-20130807PRD3]; U.S. Department of Energy by Los Alamos National Laboratory [DE-AC52-06NA25396, LA15-SignalPropogation-NDD2Ab]; US DOE's Fossil Energy-Coal Office FX We thank the RSNC for providing us with the seismic data used in this study. Additional seismic data were obtained from the FDSN via IRIS, and gravity data were obtained from the Bureau Gravimetrique International. We also thank Editor P. Shearer, as well as two anonymous reviewers, for their comments on the manuscript. This work was supported by Los Alamos National Laboratory Director's Postdoctoral fellowship LDRD-20130807PRD3, and under the auspices of the U.S. Department of Energy by Los Alamos National Laboratory under contract DE-AC52-06NA25396 and LA15-SignalPropogation-NDD2Ab. This work was also part of the U.S. Department of Energy's crosscutting initiative on subsurface science and engineering (SubTER) and was partly supported by the US DOE's Fossil Energy-Coal Office through its Carbon Capture, Utilization, and Storage Program as managed by the National Energy Technology Laboratory's Strategic Center for Coal. The views and conclusions contained in this document are those of the authors and should not be interpreted as necessarily representing the official policies, either expressed or implied, of the U.S. Government. NR 72 TC 2 Z9 2 U1 11 U2 23 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0012-821X EI 1385-013X J9 EARTH PLANET SC LETT JI Earth Planet. Sci. Lett. PD JUN 15 PY 2016 VL 444 BP 139 EP 149 DI 10.1016/j.epsl.2016.03.050 PG 11 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA DL7KE UT WOS:000375818800013 ER PT J AU Yang, X Tang, JW Mustard, JF Wu, J Zhao, KG Serbin, S Lee, JE AF Yang, Xi Tang, Jianwu Mustard, John F. Wu, Jin Zhao, Kaiguang Serbin, Shawn Lee, Jung-Eun TI Seasonal variability of multiple leaf traits captured by leaf spectroscopy at two temperate deciduous forests SO REMOTE SENSING OF ENVIRONMENT LA English DT Article DE Phenology; Leaf physiology; Foliar chemistry; Carbon cycle; Chlorophyll; Carotenoids; Nitrogen; Leaf mass per area; Partial least square regression (PLSR); Sun and shaded leaves ID PHOTOSYNTHETIC CAPACITY; TROPICAL FORESTS; IMAGING SPECTROSCOPY; CHLOROPHYLL CONTENT; NITROGEN; REFLECTANCE; PHENOLOGY; PATTERNS; LEAVES; CO2 AB Understanding the temporal patterns of leaf traits is critical in determining the seasonality and magnitude of terrestrial carbon, water, and energy fluxes. However, we lack robust and efficient ways to monitor the temporal dynamics of leaf traits. Here we assessed the potential of leaf spectroscopy to predict and monitor leaf traits across their entire life cycle at different forest sites and light environments (sunlit vs. shaded) using a weekly sampled dataset across the entire growing season at two temperate deciduous forests. The dataset includes field measured leaf-level directional-hemispherical reflectance/transmittance together with seven important leaf traits [total chlorophyll (chlorophyll a and b), carotenoids, mass-based nitrogen concentration (N-mass), mass-based carbon mass, concentration (C-mass), and leaf mass per area (LMA)]. All leaf traits varied significantly throughout the growing season, and displayed trait-specific temporal patterns. We used a Partial Least Square Regression (PLSR) modeling approach to estimate leaf traits from spectra, and found that PLSR was able to capture the variability across time, sites, and light environments of all leaf traits investigated (R-2 = 0.6-0.8 for temporal variability; R-2 = 0.3-0.7 for cross-site variability; R-2 = 0.4-0.8 for variability from light environments). We also tested alternative field sampling designs and found that for most leaf traits, biweekly leaf sampling throughout the growing season enabled accurate characterization of the seasonal patterns. Compared with the estimation of foliar pigments, the performance of N-mass, C-mass and LMA PLSR models improved more significantly with sampling frequency. Our results demonstrate that leaf spectra-trait relationships vary with time, and thus tracking the seasonality of leaf traits requires statistical models calibrated with data sampled throughout the growing season. Our results have broad implications for future research that use vegetation spectra to infer leaf traits at different growing stages. (C) 2016 Elsevier Inc. All rights reserved. C1 [Yang, Xi; Mustard, John F.; Lee, Jung-Eun] Brown Univ, Dept Earth Environm & Planetary Sci, Providence, RI 02912 USA. [Yang, Xi; Tang, Jianwu] Marine Biol Lab, Ctr Ecosyst, Woods Hole, MA 02543 USA. [Wu, Jin] Univ Arizona, Dept Ecol & Evolutionary Biol, Tucson, AZ 85721 USA. [Zhao, Kaiguang] Ohio State Univ, Ohio Agr Res & Dev Ctr, Sch Environm & Nat Resources, Wooster, OH 44691 USA. [Wu, Jin; Serbin, Shawn] Brookhaven Natl Lab, Environm & Climate Sci Dept, Upton, NY 11973 USA. RP Yang, X (reprint author), Brown Univ, Dept Earth Environm & Planetary Sci, Providence, RI 02912 USA.; Tang, JW (reprint author), Marine Biol Lab, Ctr Ecosyst, Woods Hole, MA 02543 USA. EM xi_yang@brown.edu; jtang@mbl.edu RI Tang, Jianwu/K-6798-2014; Serbin, Shawn/B-6392-2009; Zhao, Kaiguang/D-1172-2010; OI Tang, Jianwu/0000-0003-2498-9012; Serbin, Shawn/0000-0003-4136-8971; Yang, Xi/0000-0002-5095-6735 FU Brown University-Marine Biological Laboratory graduate program in Biological and Environmental Sciences; Marine Biological Laboratory; U.S. Department of Energy (DOE) Office of Biological and Environmental Research grant [DE-SC0006951]; National Science Foundation [DBI-959333, AGS-1005663]; U.S. DOE [DE-SC00112704]; NASA Earth and Space Science Fellowship (NESSF) FX We thank Katie Laushman, Lakiah Clark, Skyler Hackley, Rui Zhang, Kate Morkeski, Mengdi Cui, Marc Mayes and Tim Savas for assisting with fieldwork. We thank Matthew Erickson, Marshall Otter, Rich McHorney, Jane Tucker and Sam Kelsey from the Marine Biological Laboratory for the help with labwork. We also thank the Harvard Forest, the Manuel F. Correllus State Forest, Nature's Conservancy Hoft Farm Preserve and Mr. Colbert for the permission to use the forests for research. This research was supported by the Brown University-Marine Biological Laboratory graduate program in Biological and Environmental Sciences, and Marine Biological Laboratory start-up funding for JT. JT was also partially supported by the U.S. Department of Energy (DOE) Office of Biological and Environmental Research grant DE-SC0006951 and the National Science Foundation grants DBI-959333 and AGS-1005663. SPS was supported in part by the U.S. DOE contract No. DE-SC00112704 to Brookhaven National Laboratory. JW was supported by the NASA Earth and Space Science Fellowship (NESSF2014). NR 65 TC 1 Z9 1 U1 11 U2 42 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 0034-4257 EI 1879-0704 J9 REMOTE SENS ENVIRON JI Remote Sens. Environ. PD JUN 15 PY 2016 VL 179 BP 1 EP 12 DI 10.1016/j.rse.2016.03.026 PG 12 WC Environmental Sciences; Remote Sensing; Imaging Science & Photographic Technology SC Environmental Sciences & Ecology; Remote Sensing; Imaging Science & Photographic Technology GA DL3AH UT WOS:000375506100001 ER PT J AU Thorpe, AK Frankenberg, C Aubrey, AD Roberts, DA Nottrott, AA Rahn, TA Sauer, JA Dubey, MK Costigan, KR Arata, C Steffke, AM Hills, S Haselwimmer, C Charlesworth, D Funk, CC Green, RO Lundeen, SR Boardman, JW Eastwood, ML Sarture, CM Nolte, SH Mccubbin, IB Thompson, DR McFadden, JP AF Thorpe, A. K. Frankenberg, C. Aubrey, A. D. Roberts, D. A. Nottrott, A. A. Rahn, T. A. Sauer, J. A. Dubey, M. K. Costigan, K. R. Arata, C. Steffke, A. M. Hills, S. Haselwimmer, C. Charlesworth, D. Funk, C. C. Green, R. O. Lundeen, S. R. Boardman, J. W. Eastwood, M. L. Sarture, C. M. Nolte, S. H. Mccubbin, I. B. Thompson, D. R. McFadden, J. P. TI Mapping methane concentrations from a controlled release experiment using the next generation airborne visible/infrared imaging spectrometer (AVIRIS-NG) SO REMOTE SENSING OF ENVIRONMENT LA English DT Article DE Methane; CH4; Mapping; Concentrations; Controlled; Release; Experiment; Next generation Airborne Visible/Infrared Imaging Spectrometer; AVIRIS-NG; Fugitive; Emissions; Attribution; Monitoring; Surveys; Detection; Plumes; Point sources; Sensitivity; Fluxes ID GAS PRODUCTION SITES; MATCHED-FILTER DETECTION; UNITED-STATES; PROCESS EQUIPMENT; EMISSIONS; RETRIEVAL; QUANTIFICATION; SPECTROSCOPY AB Emissions estimates of anthropogenic methane (CH4) sources are highly uncertain and many sources related to energy production are localized yet difficult to quantify. Airborne imaging spectrometers like the next generation Airborne Visible/Infrared Imaging Spectrometer (AVIRIS-NG) are well suited for locating CH4 point sources due to their ability to map concentrations over large regions with the high spatial resolution necessary to resolve localized emissions. AVIRIS-NG was deployed during a field campaign to measure controlled CH4 releases at the Rocky Mountain Oilfield Testing Center (RMOTC) in Wyoming, U.S. for multiple flux rates and flight altitudes. Two algorithms were applied to AVIRIS-NG scenes, a matched filter detection algorithm and a hybrid retrieval approach using the Iterative Maximum a Posteriori Differential Optical Absorption Spectroscopy (IMAP-DOAS) algorithm and Singular Value Decomposition. Plumes for releases as low as 14.16 m(3)/h (0.09 kt/year) were consistently observed by AVIRIS-NG at multiple flight altitudes and images of plumes were in agreement with wind directions measured at ground stations. In some cases plumes as low as 3.40 m(3)/h (0.02 kt/year) were detected, indicating that AVIRIS-NG has the capability of detecting a wide range of fugitive CH4 source categories for natural gas fields. This controlled release experiment is the first of its kind using AVIRIS-NG and demonstrates the utility of imaging spectrometers for direct attribution of emissions to individual point source locations. This is particularly useful given the large uncertainties associated with anthropogenic CH4 emissions, including those from industry, gas transmission lines, and the oil and gas sectors. (C) 2015 Elsevier Inc. All rights reserved. C1 [Thorpe, A. K.; Frankenberg, C.; Aubrey, A. D.; Green, R. O.; Lundeen, S. R.; Eastwood, M. L.; Sarture, C. M.; Nolte, S. H.; Mccubbin, I. B.; Thompson, D. R.] CALTECH, Jet Prop Lab, Pasadena, CA USA. [Thorpe, A. K.; Roberts, D. A.; McFadden, J. P.] Univ Calif Santa Barbara, Dept Geog, Santa Barbara, CA 93106 USA. [Frankenberg, C.] CALTECH, Pasadena, CA 91125 USA. [Nottrott, A. A.] Picarro Inc, Santa Clara, CA USA. [Rahn, T. A.; Sauer, J. A.; Dubey, M. K.; Costigan, K. R.] Los Alamos Natl Lab, Los Alamos, NM USA. [Arata, C.] Univ Calif Berkeley, Dept Environm Sci Policy & Management, Berkeley, CA 94720 USA. [Steffke, A. M.; Hills, S.; Haselwimmer, C.; Charlesworth, D.] Chevron Energy Technol Co, San Ramon, CA USA. [Funk, C. C.] US Geol Survey, Santa Barbara, CA USA. [Funk, C. C.] Univ Calif Santa Barbara, Dept Geog, Climate Hazards Grp, Santa Barbara, CA 93106 USA. [Boardman, J. W.] Analyt Imaging & Geophys LLC, Boulder, CO USA. RP Thorpe, AK (reprint author), CALTECH, Jet Prop Lab, Pasadena, CA USA. EM Andrew.K.Thorpe@jpl.nasa.gov RI Dubey, Manvendra/E-3949-2010; Frankenberg, Christian/A-2944-2013; OI Dubey, Manvendra/0000-0002-3492-790X; Frankenberg, Christian/0000-0002-0546-5857; Rahn, Thomas/0000-0001-8634-1348 FU NASA Headquarters under the NASA Earth and Space Science Fellowship Program [NNX13AM95H]; Chevron Energy Technology Company FX The authors thank the AVIRIS/AVIRIS-NG team at JPL, additional collaborators at LANL, the Chevron Energy Technology Company, and the U.S. Department of Energy for use of RMOTC. Special thanks to Martin Evans, Lance Christensen, Glynn Hulley, Pierre Guillevic, and Simon Hook for their support of the project. Portions of this research were supported by NASA Headquarters under the NASA Earth and Space Science Fellowship Program grant NNX13AM95H as well as the Chevron Energy Technology Company. This work was undertaken in part at the Jet Propulsion Laboratory, California Institute of Technology, under contract with NASA as well as at the University of California, Santa Barbara. The AVIRIS-NG data used in this study are available upon request at http://avirisng.jpl.nasa.gov/ or http://aviris.jpl.nasa.gov/. Copyright 2015. All rights reserved. NR 45 TC 4 Z9 4 U1 4 U2 27 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 0034-4257 EI 1879-0704 J9 REMOTE SENS ENVIRON JI Remote Sens. Environ. PD JUN 15 PY 2016 VL 179 BP 104 EP 115 DI 10.1016/j.rse.2016.03.032 PG 12 WC Environmental Sciences; Remote Sensing; Imaging Science & Photographic Technology SC Environmental Sciences & Ecology; Remote Sensing; Imaging Science & Photographic Technology GA DL3AH UT WOS:000375506100009 ER PT J AU Qu, J Cooley, KM Shawa, AH Lu, RY Blau, PJ AF Qu, Jun Cooley, Kevin M. Shawa, Austin H. Lu, Roger Y. Blau, Peter J. TI Assessment of wear coefficients of nuclear zirconium claddings without and with pre-oxidation SO WEAR LA English DT Article DE Grid-to-rod-fretting (GTRF); Nuclear zirconium claddings; Wear coefficient; Pre-oxidation; Stage-wise wear model ID FRETTING-WEAR; BEHAVIOR; ALLOYS AB In the cores of pressurized water nuclear reactors, water-flow induced vibration is known to cause claddings on the fuel rods to rub against their supporting grids. Such grid-to-rod-fretting (GTRF) may lead to fretting wear-through and the leakage of radioactive species. The surfaces of actual zirconium alloy claddings in a reactor are inevitably oxidized in the high-temperature pressurized water, and some claddings are even pre-oxidized. As a result, the wear process of the surface oxide film is expected to be quite different from the zirconium alloy substrate. This study attempts to measure the wear coefficients of zirconium claddings without and with pre-oxidation rubbing against grid samples using a bench-scale fretting tribometer. Results suggest that the volumetric wear coefficient of the pre-oxidized cladding is 50 to 200 times lower than that of the untreated cladding. In terms of the linear rate of wear depth, the pre-oxidized alloy wears about 15 times more slowly than the untreated cladding. Fitted with the experimentally-determined wear rates, a stage-wise GTRF engineering wear model demonstrates good agreement with in-reactor experience in predicting the trend of cladding lives. (C) 2016 Elsevier B.V. All rights reserved. C1 [Qu, Jun; Cooley, Kevin M.; Shawa, Austin H.] Oak Ridge Natl Lab, Mat Sci & Technol Div, POB 2008,MS-6063, Oak Ridge, TN 37831 USA. [Lu, Roger Y.] Westinghouse Elect Co, 5801 Bluff Rd, Hopkins, SC 29061 USA. [Blau, Peter J.] Blau Tribol Consulting, Enka, NC 28728 USA. RP Qu, J (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, POB 2008,MS-6063, Oak Ridge, TN 37831 USA. EM qujn@ornl.gov OI Qu, Jun/0000-0001-9466-3179 FU Consortium for Advanced Simulation of Light Water Reactors; Energy Innovation Hub FX This research was supported by the Consortium for Advanced Simulation of Light Water Reactors (http://www.casi.gov), an Energy Innovation Hub (http://www.energy.gov/hubs) for Modeling and Simulation of Nuclear Reactors, U.S. Department of Energy. The authors thank Randy J. Parten and William C. Barnhill from ORNL for fretting machine modification and assistance on wear volume quantification, respectively. NR 23 TC 2 Z9 2 U1 4 U2 8 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0043-1648 EI 1873-2577 J9 WEAR JI Wear PD JUN 15 PY 2016 VL 356-357 BP 17 EP 22 DI 10.1016/j.wear.2016.02.020 PG 6 WC Engineering, Mechanical; Materials Science, Multidisciplinary SC Engineering; Materials Science GA DL7TP UT WOS:000375843300003 ER PT J AU Zhang, YL Shen, YT Chen, Y Yan, YS Pan, JM Xiong, QG Shi, WD Yu, LB AF Zhang, Yunlei Shen, Yating Chen, Yao Yan, Yongsheng Pan, Jianming Xiong, Qingang Shi, Weidong Yu, Longbao TI Hierarchically carbonaceous catalyst with Bronsted-Lewis acid sites prepared through Pickering HIPEs templating for biomass energy conversation SO CHEMICAL ENGINEERING JOURNAL LA English DT Article DE Cellulose conversion; 5-Hydroxymethylfurfural; Hierarchically porous structures; Bronsted-Lewis acid sites; High internal phase emulsions templating ID INTERNAL PHASE EMULSIONS; MESOPOROUS SILICA NANOPARTICLES; TO-HMF CONVERSION; ONE-POT CELLULOSE; IONIC LIQUID; LIGNOCELLULOSIC BIOMASS; HETEROGENEOUS CATALYSIS; RECYCLABLE CATALYST; AMORPHOUS-CARBON; POROUS STRUCTURE AB In this study, macroporous inorganic-organic hybrid polymers (MIPs) were prepared using versatile high internal phase emulsions (HIPEs) templating to synthesize a novel catalyst for cellulose conversion. Upon the incomplete hydrothermal carbonization of MIPs and sulfonation with H2SO4, macroporous carbonaceous solid catalysts (MCSC) with hierarchical structures and Brensted-Lewis acid sites were obtained. The synthesized MCSC was found to be highly effective to produce 5-hydroxymethylfurfural (HMF) in the 1-butyl-3-methyl-imidazolium chloride ([BMIM]-Cl) ionic liquids. It was shown that remarkable HMF yield (43.1%) and selectivity (57.7%) can be obtained and the catalyst is recyclable up to four consecutive cycles without significant loss of catalytic activity. This implies that catalysts with designed physicochemical characteristics are advantageous over traditional ones in producing HMF. A catalytic scheme was proposed to characterize the cellulose conversion to HMF using the MCSC. (C) 2016 Elsevier B.V. All rights reserved. C1 [Zhang, Yunlei; Shen, Yating; Yan, Yongsheng; Pan, Jianming; Shi, Weidong; Yu, Longbao] Jiangsu Univ, Sch Chem & Chem Engn, Zhenjiang 212013, Peoples R China. [Chen, Yao] Jiangsu Univ, Sch Environm & Safety Engn, Zhenjiang 212013, Peoples R China. [Xiong, Qingang] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Yan, YS; Pan, JM (reprint author), Jiangsu Univ, Sch Chem & Chem Engn, Zhenjiang 212013, Peoples R China.; Xiong, QG (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. EM jdxz2011@126.com; zhenjiangpjm@126.com; xiongq@ornl.gov FU National Natural Science Foundation of China [21107037, 21176107, 21306013]; Natural Science Foundation of Jiangsu Province [BK2011461, BK2011514]; National Postdoctoral Science Foundation [2013M530240]; Postdoctoral Science Foundation of Jiangsu Province [1202002B]; Programs of Senior Talent Foundation of Jiangsu University [12JDG090] FX This work was financially supported by the National Natural Science Foundation of China (Nos. 21107037, 21176107 and 21306013), Natural Science Foundation of Jiangsu Province (Nos. BK2011461 and BK2011514), National Postdoctoral Science Foundation (No. 2013M530240), Postdoctoral Science Foundation funded Project of Jiangsu Province (No. 1202002B) and Programs of Senior Talent Foundation of Jiangsu University (No. 12JDG090). NR 63 TC 5 Z9 5 U1 30 U2 91 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 1385-8947 EI 1873-3212 J9 CHEM ENG J JI Chem. Eng. J. PD JUN 15 PY 2016 VL 294 BP 222 EP 235 DI 10.1016/j.cej.2016.02.092 PG 14 WC Engineering, Environmental; Engineering, Chemical SC Engineering GA DK8IK UT WOS:000375170200024 ER PT J AU Niu, C Shi, XY Liu, FD Liu, K Xie, LJ You, Y He, H AF Niu, Can Shi, Xiaoyan Liu, Fudong Liu, Kuo Xie, Lijuan You, Yan He, Hong TI High hydrothermal stability of Cu-SAPO-34 catalysts for the NH3-SCR of NOx SO CHEMICAL ENGINEERING JOURNAL LA English DT Article DE Cu-SAPO-34; NH3-SCR; Hydrothermal stability; Copper species ID ONE-POT SYNTHESIS; CALCINATION-TEMPERATURE; ACTIVE-SITES; CU/SAPO-34 CATALYSTS; MONOLITH CATALYST; DIESEL VEHICLES; REDUCTION SCR; NH3; ZEOLITE; PERFORMANCE AB The effects of calcination temperature, Cu source and co-template contents on the activity and hydrothermal stability of Cu-SAPO-34 catalysts prepared by the one-pot hydrothermal synthesis method were investigated. Appropriate calcination temperature was important for the deNOx activity of Cu-SAPO-34 catalyst. The amount of Cu source and co-template in the resulting gel could impact the Cu loading and the crystallization of the final Cu-SAPO-34. Preferably, hydrothermal treatment of the Cu-SAPO-34 catalyst with Cu loading ca. 3.44% at 750 degrees C for 16 h increased the NH3-SCR activity slightly due to migration of CuO to isolated Cu2+ and the maintenance of the crystallinity as well as the acidity. Moreover, the catalyst aged at 800 degrees C for 16 h maintained >90% NOx conversion from 225 to 400 degrees C, and the crystallinity, active Cu2+ species and acidity in Cu-SAPO-34 were not destroyed completely after such harsh treatment. Meanwhile, kinetic analysis over fresh and aged Cu-SAPO-34 samples were conducted and the conclusion were in agreement with the NH3-SCR tests, H-2-TPR and NH3-TPD results. (C) 2016 Elsevier B.V. All rights reserved. C1 [Niu, Can; Shi, Xiaoyan; Liu, Fudong; Liu, Kuo; Xie, Lijuan; You, Yan; He, Hong] Chinese Acad Sci, State Key Joint Lab Environm Simulat & Pollut Con, Ecoenvironm Sci Res Ctr, 18 ShuangQing Rd, Beijing 100085, Peoples R China. [Liu, Fudong] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP You, Y; He, H (reprint author), Chinese Acad Sci, State Key Joint Lab Environm Simulat & Pollut Con, Ecoenvironm Sci Res Ctr, 18 ShuangQing Rd, Beijing 100085, Peoples R China. EM yanyou@rcees.ac.cn; honghe@rcees.ac.cn FU National Natural Science Foundation of China [51278486, 51578536, 21303247] FX This work was financially supported by the National Natural Science Foundation of China (51278486, 51578536, 21303247). NR 47 TC 6 Z9 6 U1 42 U2 102 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 1385-8947 EI 1873-3212 J9 CHEM ENG J JI Chem. Eng. J. PD JUN 15 PY 2016 VL 294 BP 254 EP 263 DI 10.1016/j.cej.2016.02.086 PG 10 WC Engineering, Environmental; Engineering, Chemical SC Engineering GA DK8IK UT WOS:000375170200027 ER PT J AU Das, S Maroli, A Singh, SS Stannard, T Xiao, XH Chawla, N Neithalath, N AF Das, Sumanta Maroli, Amit Singh, Sudhanshu S. Stannard, Tyler Xiao, Xianghui Chawla, Nikhilesh Neithalath, Narayanan TI A microstructure-guided constitutive modeling approach for random heterogeneous materials: Application to structural binders SO COMPUTATIONAL MATERIALS SCIENCE LA English DT Article DE Microstructure; Constitutive model; Finite element; X-ray tomography; Nanoindentation; Binders ID RAY SYNCHROTRON TOMOGRAPHY; HIGH-PERFORMANCE CONCRETE; BOUNDARY-CONDITIONS; ELASTIC PROPERTIES; SELF-CONSISTENT; MICRO STRUCTURE; CEMENT PASTE; COMPUTATIONAL HOMOGENIZATION; REPRESENTATIVE VOLUME; MECHANICAL-BEHAVIOR AB This paper presents a microstructure-guided modeling approach to predict the effective elastic response of heterogeneous materials, and demonstrates its application toward two highly heterogeneous, unconventional structural binders, i.e., iron carbonate and fly ash geopolymer. Microstructural information from synchrotron X-ray tomography (XRT) and intrinsic elastic properties of component solid phases from statistical nanoindentation are used as the primary inputs. The virtual periodic 3D microstructure reconstructed using XRT, along with periodic boundary conditions is used as a basis for strain-controlled numerical simulation scheme in the linear elastic range to predict the elastic modulus as well as the stresses in the microstructural phases. The elastic modulus of the composite material predicted from the microstructure-based constitutive modeling approach correlates very well with experimental measurements for both the materials considered. This technique efficiently links the microstructure to mechanical properties of interest and helps develop material design guidelines for novel heterogeneous composites. (C) 2016 Elsevier B.V. All rights reserved. C1 [Das, Sumanta; Maroli, Amit; Neithalath, Narayanan] Arizona State Univ, Sch Sustainable Engn & Built Environm, Tempe, AZ USA. [Singh, Sudhanshu S.; Stannard, Tyler; Chawla, Nikhilesh] Arizona State Univ, Mat Sci & Engn, Tempe, AZ USA. [Xiao, Xianghui] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Singh, Sudhanshu S.] Indian Inst Technol, Dept Mat Sci & Engn, Kanpur 208016, Uttar Pradesh, India. RP Neithalath, N (reprint author), Arizona State Univ, Sch Sustainable Engn & Built Environm, Tempe, AZ USA. EM Narayanan.Neithalath@asu.edu FU National Science Foundation (NSF) [CMMI: 1068985, CMMI: 1353170] FX The authors gratefully acknowledge the National Science Foundation (NSF) for the support for this research (CMMI: 1068985 and CMMI: 1353170). This research was conducted in the Laboratory for the Science of Sustainable Infrastructural Materials, the Structural Engineering Laboratory, 4D Materials Science Laboratory, and LeRoy Eyring Center for Solid State Science at Arizona State University and the supports that have made these laboratories possible are acknowledged. The 2-BM beamline of the Advanced Photon Source (APS) at Argonne National Laboratory is also acknowledged. The contents of this paper reflect the views of the authors who are responsible for the facts and accuracy of the data presented herein, and do not necessarily reflect the views and policies of the funding agency, nor do the contents constitute a standard, specification, or a regulation. NR 69 TC 2 Z9 2 U1 2 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0927-0256 EI 1879-0801 J9 COMP MATER SCI JI Comput. Mater. Sci. PD JUN 15 PY 2016 VL 119 BP 52 EP 64 DI 10.1016/j.commatsci.2016.03.040 PG 13 WC Materials Science, Multidisciplinary SC Materials Science GA DK6YD UT WOS:000375070800008 ER PT J AU Bao, F Archibald, R Bansal, D Delaire, O AF Bao, Feng Archibald, Rick Bansal, Dipanshu Delaire, Olivier TI Hierarchical optimization for neutron scattering problems SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Neutron scattering; Model reduction; Global optimization; Stochastic; Confidence distribution AB We present a scalable optimization method for neutron scattering problems that determines confidence regions of simulation parameters in lattice dynamics models used to fit neutron scattering data for crystalline solids. The method uses physics-based hierarchical dimension reduction in both the computational simulation domain and the parameter space. We demonstrate for silicon that after a few iterations the method converges to parameters values (interatomic force-constants) computed with density functional theory simulations. Published by Elsevier Inc. C1 [Bao, Feng; Archibald, Rick] Oak Ridge Natl Lab, Div Math & Comp Sci, One Bethel Valley Rd,POB 2008,MS-6211, Oak Ridge, TN 37831 USA. [Bansal, Dipanshu; Delaire, Olivier] Oak Ridge Natl Lab, Div Mat Sci & Technol, One Bethel Valley Rd,POB 2008,MS-6118, Oak Ridge, TN 37831 USA. RP Archibald, R (reprint author), Oak Ridge Natl Lab, Div Math & Comp Sci, One Bethel Valley Rd,POB 2008,MS-6211, Oak Ridge, TN 37831 USA. EM archibaldrk@ornl.gov RI Archibald, Rick/I-6238-2016; Bansal, Dipanshu/I-7895-2016 OI Archibald, Rick/0000-0002-4538-9780; Bansal, Dipanshu/0000-0003-1181-1119 FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division, through the Office of Science Early Career Research Program; Advanced Scientific Computing Research, through the ACUMEN project FX Acknowledges support by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division, through the Office of Science Early Career Research Program and Advanced Scientific Computing Research, through the ACUMEN project. NR 19 TC 1 Z9 1 U1 1 U2 3 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD JUN 15 PY 2016 VL 315 BP 39 EP 51 DI 10.1016/j.jcp.2016.03.017 PG 13 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA DK3QO UT WOS:000374832700003 ER PT J AU Saye, RI Sethian, JA AF Saye, R. I. Sethian, J. A. TI Multiscale modelling of evolving foams SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Foams; Voronoi Implicit Interface Methods; Multiscale multiphysics; Interface dynamics; Bubbles; Thin-film equations ID PARTIAL-DIFFERENTIAL-EQUATIONS; LEVEL SET METHODS; IMPLICIT INTERFACE METHOD; NAVIER-STOKES EQUATIONS; SINGLE PLATEAU BORDERS; SURFACE-TENSION; PROPAGATING INTERFACES; THIN-FILMS; DRAINAGE; FLOW AB We present a set of multi-scale interlinked algorithms to model the dynamics of evolving foams. These algorithms couple the key effects of macroscopic bubble rearrangement, thin film drainage, and membrane rupture. For each of the mechanisms, we construct consistent and accurate algorithms, and couple them together to work across the wide range of space and time scales that occur in foam dynamics. These algorithms include second order finite difference projection methods for computing incompressible fluid flow on the macroscale, second order finite element methods to solve thin film drainage equations in the lamellae and Plateau borders, multiphase Voronoi Implicit Interface Methods to track interconnected membrane boundaries and capture topological changes, and Lagrangian particle methods for conservative liquid redistribution during rearrangement and rupture. We derive a full set of numerical approximations that are coupled via interface jump conditions and flux boundary conditions, and show convergence for the individual mechanisms. We demonstrate our approach by computing a variety of foam dynamics, including coupled evolution of three-dimensional bubble clusters attached to an anchored membrane and collapse of a foam cluster. (C) 2016 Elsevier Inc. All rights reserved. C1 [Sethian, J. A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. Univ Calif Berkeley, Dept Math, Berkeley, CA 94720 USA. RP Sethian, JA (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM sethian@math.berkeley.edu FU Applied Mathematics Program of U.S. DOE Office of Advanced Scientific Computing Research [DE-AC02-05CH11231]; Division of Mathematical Sciences of National Science Foundation [1319276]; Office of Science of U.S. DOE [DE-AC02-05CH11231]; Miller Foundation at University of California, Berkeley; American Australian Association Sir Keith Murdoch Fellowship; Luis W. Alvarez Postdoctoral Fellowship; Einstein Visiting Fellow of the Einstein Stiftung Berlin FX This research was supported in part by the Applied Mathematics Program of the U.S. DOE Office of Advanced Scientific Computing Research under contract number DE-AC02-05CH11231 and by the Division of Mathematical Sciences of the National Science Foundation, grant number 1319276. Some computations used the resources of the National Energy Research Scientific Computing Center (NERSC), which is supported by the Office of Science of the U.S. DOE under Contract No. DE-AC02-05CH11231. J.S. was also supported by the Miller Foundation at University of California, Berkeley, and as an Einstein Visiting Fellow of the Einstein Stiftung Berlin. R.S. was also supported by an American Australian Association Sir Keith Murdoch Fellowship and a Luis W. Alvarez Postdoctoral Fellowship. NR 57 TC 1 Z9 1 U1 9 U2 20 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD JUN 15 PY 2016 VL 315 BP 273 EP 301 DI 10.1016/j.jcp.2016.02.077 PG 29 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA DK3QO UT WOS:000374832700017 ER PT J AU Ku, S Hager, R Chang, CS Kwon, JM Parker, SE AF Ku, S. Hager, R. Chang, C. S. Kwon, J. M. Parker, S. E. TI A new hybrid-Lagrangian numerical scheme for gyrokinetic simulation of tokamak edge plasma SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Plasma; Tokamak; Gyrokinetic; Lagrangian; delta-f; XGC ID PARTICLE-IN-CELL; TURBULENCE; RESOLUTION; MODEL AB In order to enable kinetic simulation of non-thermal edge plasmas at a reduced computational cost, a new hybrid-Lagrangian delta f scheme has been developed that utilizes the phase space grid in addition to the usual marker particles, taking advantage of the computational strengths from both sides. The new scheme splits the particle distribution function of a kinetic equation into two parts. Marker particles contain the fast space-time varying, delta f, part of the distribution function and the coarse-grained phase-space grid contains the slow space-time varying part. The coarse-grained phase-space grid reduces the memory-requirement and the computing cost, while the marker particles provide scalable computing ability for the fine-grained physics. Weights of the marker particles are determined by a direct weight evolution equation instead of the differential form weight evolution equations that the conventional delta-f schemes use. The particle weight can be slowly transferred to the phase space grid, thereby reducing the growth of the particle weights. The non-Lagrangian part of the kinetic equation - e.g., collision operation, ionization, charge exchange, heat-source, radiative cooling, and others - can be operated directly on the phase space grid. Deviation of the particle distribution function on the velocity grid from a Maxwellian distribution function - driven by ionization, charge exchange and wall loss - is allowed to be arbitrarily large. The numerical scheme is implemented in the gyrokinetic particle code XGC1, which specializes in simulating the tokamak edge plasma that crosses the magnetic separatrix and is in contact with the material wall. (C) 2016 Elsevier Inc. All rights reserved. C1 [Ku, S.; Hager, R.; Chang, C. S.] Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. [Kwon, J. M.] Natl Fus Res Inst, Daejeon, South Korea. [Parker, S. E.] Univ Colorado Boulder, Boulder, CO USA. RP Ku, S (reprint author), Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08543 USA. EM sku@pppl.gov RI Ku, Seung-Hoe/D-2315-2009 OI Ku, Seung-Hoe/0000-0002-9964-1208 FU U.S. Department of Energy [DE-AC02-09CH11466, DE-SC000801]; Office of Science of the U.S. Department of Energy [DE-AC05-00OR22725] FX This work was supported by the U.S. Department of Energy under Contract No. DE-AC02-09CH11466 and Grant No. DE-SC000801. This work used resources of the Oak Ridge Leadership Computing Facility at the Oak Ridge National Laboratory, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC05-00OR22725. NR 22 TC 1 Z9 1 U1 5 U2 8 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD JUN 15 PY 2016 VL 315 BP 467 EP 475 DI 10.1016/j.jcp.2016.03.062 PG 9 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA DK3QO UT WOS:000374832700026 ER PT J AU Hager, R Yoon, ES Ku, S D'Azevedo, EF Worley, PH Chang, CS AF Hager, Robert Yoon, E. S. Ku, S. D'Azevedo, E. F. Worley, P. H. Chang, C. S. TI A fully non-linear multi-species Fokker-Planck-Landau collision operator for simulation of fusion plasma SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Plasma; Fusion; Collision operator; XGC; Particle-in-cell ID TRANSPORT; EQUATION AB Fusion edge plasmas can be far from thermal equilibrium and require the use of a non-linear collision operator for accurate numerical simulations. In this article, the non-linear single-species Fokker-Planck-Landau collision operator developed by Yoon and Chang (2014) [9] is generalized to include multiple particle species. The finite volume discretization used in this work naturally yields exact conservation of mass, momentum, and energy. The implementation of this new non-linear Fokker-Planck-Landau operator in the gyrokinetic particle-in-cell codes XGC1 and XGCa is described and results of a verification study are discussed. Finally, the numerical techniques that make our non-linear collision operator viable on high-performance computing systems are described, including specialized load balancing algorithms and nested OpenMP parallelization. The collision operator's good weak and strong scaling behavior are shown. (C) 2016 Elsevier Inc. All rights reserved. C1 [Hager, Robert; Ku, S.; Chang, C. S.] Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA. [Yoon, E. S.] Rensselaer Polytech Inst, 110 8th St, Troy, NY 12180 USA. [D'Azevedo, E. F.; Worley, P. H.] Oak Ridge Natl Lab, POB 2008, Oak Ridge, TN 37831 USA. RP Hager, R (reprint author), Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA. EM rhager@pppl.gov; yoone@rpi.edu; sku@pppl.gov; dazevedoef@ornl.gov; worleyph@ornl.gov; cschang@pppl.gov RI Ku, Seung-Hoe/D-2315-2009 OI Ku, Seung-Hoe/0000-0002-9964-1208 FU Scientific Discovery through Advanced Computing (SciDAC) program - U.S. Department of Energy Office of Advanced Scientific Computing Research and the Office of Fusion Energy Sciences [DE-AC02-09CH11466]; Princeton University [DE-AC02-09CH11466]; UT-Battelle, LLC [De-AC05-00OR22725]; Rensselaer Polytechnic Institute [DE-SC0008449]; DOE Office of Science User Facility [De-AC05-00OR22725, DE-AC02-06CH11357]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX Support for this work was provided through the Scientific Discovery through Advanced Computing (SciDAC) program funded by the U.S. Department of Energy Office of Advanced Scientific Computing Research and the Office of Fusion Energy Sciences (DE-AC02-09CH11466). The work was performed at Princeton Plasma Physics Laboratory, which is managed by Princeton University under Contract No. DE-AC02-09CH11466, at Oak Ridge National Laboratory, which is managed by UT-Battelle, LLC under Contract No. De-AC05-00OR22725, and at Rensselaer Polytechnic Institute under Contract No. DE-SC0008449. Awards of computer time was provided by the Innovative and Novel Computational Impact on Theory and Experiment (INCITE) program. This research used resources of the Argonne Leadership Computing Facility, which is a DOE Office of Science User Facility supported under contract DE-AC02-06CH11357. This research also used resources of the Oak Ridge Leadership Computing Facility, which is a DOE Office of Science User Facility supported under Contract DE-AC05-00OR22725. This research also used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 23 TC 4 Z9 4 U1 1 U2 3 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD JUN 15 PY 2016 VL 315 BP 644 EP 660 DI 10.1016/j.jcp.2016.03.064 PG 17 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA DK3QO UT WOS:000374832700034 ER PT J AU de Castro, AR Oostrom, M Shokri, N AF de Castro, Antonio Rodriguez Oostrom, Mart Shokri, Nima TI Effects of shear-thinning fluids on residual oil formation in microfluidic pore networks SO JOURNAL OF COLLOID AND INTERFACE SCIENCE LA English DT Article DE Shear-thinning fluids; Microfluidic analysis; Polymer flooding; Oil recovery; Immiscible displacement ID REMEDIAL AMENDMENT DELIVERY; POROUS-MEDIA; POLYMER-SOLUTIONS; 2-PHASE FLOW; XANTHAN GUM; RHEOLOGICAL BEHAVIOR; VISCOUS OIL; RECOVERY; PERCOLATION; SCALE AB Two-phase immiscible displacement in porous media is controlled by capillary and viscous forces when gravitational effects are negligible. The relative importance of these forces is quantified through the dimensionless capillary number Ca and the viscosity ratio M between fluid phases. When the displacing fluid is Newtonian, the effects of Ca and M on the displacement patterns can be evaluated independently. However, when the injecting fluids exhibit shear-thinning viscosity behaviour the values of M and Ca are interdependent. Under these conditions, the effects on phase entrapment and the general displacement dynamics cannot be dissociated. In the particular case of shear-thinning aqueous polymer solutions, the degree of interdependence between M and Ca is determined by the polymer concentration. In this work, two-phase immiscible displacement experiments were performed in micromodels, using shear-thinning aqueous polymer solutions as displacing fluids, to investigate the effect of polymer concentration on the relationship between Ca and M, the recovery efficiency, and the size distribution of the trapped non wetting fluid. Our results show that the differences in terms of magnitude and distribution of the trapped phase are related to the polymer concentration which influences the values of Ca and M. (C) 2016 Elsevier Inc. All rights reserved. C1 [de Castro, Antonio Rodriguez; Shokri, Nima] Univ Manchester, Sch Chem Engn & Analyt Sci, Room C26,Sackville St, Manchester M13 9PL, Lancs, England. [Oostrom, Mart] Pacific NW Natl Lab, Energy & Environm Div, Richland, WA 99352 USA. RP Shokri, N (reprint author), Univ Manchester, Sch Chem Engn & Analyt Sci, Room C26,Sackville St, Manchester M13 9PL, Lancs, England. EM nima.shokri@manchester.ac.uk FU Royal Society [RG140088]; American Chemical Society Petroleum Research Fund [52054-DNI6] FX Nima Shokri would like to acknowledge the donors of the American Chemical Society Petroleum Research Fund for support of this research (PRF No. 52054-DNI6) and the equipment funding from The Royal Society (RG140088). We thank Nikolaos Karadimitriou who designed the micromodel. The micromodel was fabricated in the William R. Wiley Environmental Molecular Sciences Laboratory, a U.S. Department of Energy scientific user facility operated by Pacific Northwest National Laboratory. NR 61 TC 4 Z9 4 U1 6 U2 12 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9797 EI 1095-7103 J9 J COLLOID INTERF SCI JI J. Colloid Interface Sci. PD JUN 15 PY 2016 VL 472 BP 34 EP 43 DI 10.1016/j.jcis.2016.03.027 PG 10 WC Chemistry, Physical SC Chemistry GA DK0RT UT WOS:000374620600004 ER PT J AU Kim, MY Kyriakidou, EA Choi, JS Toops, TJ Binder, AJ Thomas, C Parks, JE Schwartz, V Chen, JH Hensley, DK AF Kim, Mi-Young Kyriakidou, Eleni A. Choi, Jae-Soon Toops, Todd J. Binder, Andrew J. Thomas, Cyril Parks, James E., II Schwartz, Viviane Chen, Jihua Hensley, Dale K. TI Enhancing low-temperature activity and durability of Pd-based diesel oxidation catalysts using ZrO2 supports SO APPLIED CATALYSIS B-ENVIRONMENTAL LA English DT Article DE Diesel oxidation catalyst; Palladium; Zirconia; Support; Sol-gel ID CO OXIDATION; AUTOMOTIVE EXHAUST; PERFORMANCE; DEACTIVATION; ZIRCONIA; SURFACE; OXIDES AB We investigated the impact of ZrO2 on the performance of palladium-based oxidation catalysts with respect to low-temperature activity, hydrothermal stability, and sulfur tolerance. Pd supported on ZrO2 and SiO2 were synthesized for a comparative study. Additionally, in an attempt to maximize the ZrO2 surface area and improve sulfur tolerance, a Pd support with ZrO2-dispersed onto SiO2 was studied. The physicochemical properties of the catalysts were examined using ICP, N-2 sorption, XRD, SEM, TEM, and NH3-, CO2-, and NOx-TPD. The activity of the Pd catalysts were measured from 60 to 600 degrees C in a flow of 4000 ppm CO, 500 ppm NO, 1000 ppm C3H6, 4% O-2, 5% H2O, and Ar balance. The Pd catalysts were evaluated in fresh, sulfated, and hydrothermally aged states. Overall, the ZrO2-containing catalysts showed considerably higher CO and C3H6 oxidation activity than Pd/SiO2 under the reaction conditions studied. The good performance of ZrO2-containing catalysts appeared to be due in part to high Pd dispersion resulting from strong Pd and support interaction. Another beneficial effect of strong interaction between Pd and ZrO2 was manifested as a greater hydrothermal stability with good oxidation activity even after aging at 800 and 900 degrees C for 16 h. In contrast, Pd/SiO2 suffered significant performance loss due to Pd particle coarsening. Although the Pd/ZrO2-SiO2 catalyst was not more active than Pd/ZrO2, improved tolerance to sulfur was realized. Unlike the bulk ZrO2 support, the ZrO2-incorporated SiO2 presented only weak basicity leading to a superior sulfur tolerance of Pd/ZrO2-SiO2. These results confirmed the potential of developing Pd-based oxidation catalysts with enhanced low-temperature activity and durability using ZrO2-SiO2 supports. Controlling morphology and accessible area of the dispersed ZrO2 layer appeared critical to further maximize the catalytic performance. (C) 2016 Elsevier B.V. All rights reserved. C1 [Kim, Mi-Young; Kyriakidou, Eleni A.; Choi, Jae-Soon; Toops, Todd J.; Binder, Andrew J.; Parks, James E., II] Oak Ridge Natl Lab, Fuels Engines & Emiss Res Ctr, Oak Ridge, TN USA. [Thomas, Cyril] Univ Paris 06, Sorbonne Univ, Lab React Surface, UMR 7197, 4 Pl Jussieu,Case 178, F-75252 Paris, France. [Thomas, Cyril] CNRS, Lab React Surface, UMR 7197, 4 Pl Jussieu,Case 178, F-75252 Paris, France. [Schwartz, Viviane; Chen, Jihua; Hensley, Dale K.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN USA. [Kim, Mi-Young] Heesung Catalysts, 91 Somanggongwon Ro, Siheung Si 429848, Gyeonggi Do, South Korea. RP Choi, JS (reprint author), Oak Ridge Natl Lab, Fuels Engines & Emiss Res Ctr, Oak Ridge, TN USA. EM choijs@ornl.gov RI Kyriakidou, Eleni/H-9785-2016; Chen, Jihua/F-1417-2011; OI Kyriakidou, Eleni/0000-0003-1094-0162; Chen, Jihua/0000-0001-6879-5936; Thomas, Cyril/0000-0003-4224-6095; Binder, Andrew/0000-0003-3221-2887; Choi, Jae-Soon/0000-0002-8162-4207 FU U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Vehicle Technologies Office; French National Centre for Scientific Research FX This research was sponsored by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Vehicle Technologies Office (Program Managers: Gurpreet Singh, Ken Howden and Leo Breton) and French National Centre for Scientific Research. A portion of this research including the microscopy experiments was conducted at ORNL's Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. We thank Saint-Gobain for providing the zirconia sample. NR 31 TC 1 Z9 2 U1 22 U2 92 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0926-3373 EI 1873-3883 J9 APPL CATAL B-ENVIRON JI Appl. Catal. B-Environ. PD JUN 15 PY 2016 VL 187 BP 181 EP 194 DI 10.1016/j.apcatb.2016.01.023 PG 14 WC Chemistry, Physical; Engineering, Environmental; Engineering, Chemical SC Chemistry; Engineering GA DG2ZO UT WOS:000371939500021 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Asilar, E Bergauer, T Brandstetter, J Brondolin, E Dragicevic, M Ero, J Flechl, M Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Knunz, V Konig, A Krammer, M Kratschmer, I Liko, D Matsushita, T Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schieck, J Schofbeck, R Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Lauwers, J Luyckx, S De Klundert, MV Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Abu Zeid, S Blekman, F D'Hondt, J Daci, N De Bruyn, I Deroover, K Heracleous, N Keaveney, J Lowette, S Moreels, L Olbrechts, A Python, Q Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Van Parijs, I Barria, P Brun, H Caillol, C Clerbaux, B De Lentdecker, G Fasanella, G Favart, L Grebenyuk, A Karapostoli, G Lenzi, T Leonard, A Maerschalk, T Marinov, A Pernie, L Randle-Conde, A Reis, T Seva, T Vander Velde, C Vanlaer, P Yonamine, R Zenoni, F Zhang, F Beernaert, K Benucci, L Cimmino, A Crucy, S Dobur, D Fagot, A Garcia, G Gul, M Mccartin, J Rios, AAO Poyraz, D Ryckbosch, D Salva, S Sigamani, M Strobbe, N Tytgat, M Van Driessche, W Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bondu, O Brochet, S Bruno, G Caudron, A Ceard, L Da Silveira, GG Delaere, C Favart, D Forthomme, L Giammanco, A Hollar, J Jafari, A Jez, P Komm, M Lemaitre, V Mertens, A Musich, M Nuttens, C Perrini, L Pin, A Piotrzkowski, K Popov, A Quertenmont, L Selvaggi, M Marono, MV Beliy, N Hammad, GH Alda, WL Alves, FL Alves, GA Brito, L Martins, MC Hamer, M Hensel, C Herrera, CM Moraes, A Pol, ME Teles, PR Das Chagas, EBB Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD De Souza, SF Guativa, LMH Malbouisson, H Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santoro, A Sznajder, A Manganote, EJT Pereira, AV Ahuja, S Bernardes, CA Santos, ADS Dogra, S Tomei, TRFP Gregores, EM Mercadante, PG Moon, CS Novaes, SF Padula, SS Abad, DR Vargas, JCR Aleksandrov, A Hadjiiska, R Iaydjiev, P Rodozov, M Stoykova, S Sultanov, G Vutova, M Dimitrov, A Glushkov, I Litov, L Pavlov, B Petkov, P Ahmad, M Bian, JG Chen, GM Chen, HS Chen, M Cheng, T Du, R Jiang, CH Plestina, R Romeo, F Shaheen, SM Spiezia, A Tao, J Wang, C Wang, Z Zhang, H Asawatangtrakuldee, C Ban, Y Li, Q Liu, S Mao, Y Qian, SJ Wang, D Xu, Z Avila, C Cabrera, A Sierra, LFC Florez, C Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Puljak, I Cipriano, PMR Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Micanovic, S Sudic, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Rykaczewski, H Bodlak, M Finger, M Finger, M Assran, Y Elgammal, S Kamel, AE Mahmoud, MA Mohammed, Y Calpas, B Kadastik, M Murumaa, M Raidal, M Tiko, A Veelken, C Eerola, P Pekkanen, J Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E Wendland, L Talvitie, J Tuuva, T Besancon, M Couderc, F Dejardin, M Denegri, D Fabbro, B Faure, JL Favaro, C Ferri, F Ganjour, S Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Machet, M Malcles, J Rander, J Rosowsky, A Titov, M Zghiche, A Antropov, I Baffioni, S Beaudette, F Busson, P Cadamuro, L Chapon, E Charlot, C Dahms, T Davignon, O Filipovic, N Florent, A de Cassagnac, RG Lisniak, S Mastrolorenzo, L Mine, P Naranjo, IN Nguyen, M Ochando, C Ortona, G Paganini, P Pigard, P Regnard, S Salerno, R Sauvan, JB Sirois, Y Strebler, T Yilmaz, Y Zabi, A Agram, JL Andrea, J Aubin, A Bloch, D Brom, JM Buttignol, M Chabert, EC Chanon, N Collard, C Conte, E Coubez, X Fontaine, JC Gele, D Goerlach, U Goetzmann, C Le Bihan, AC Merlin, JA Skovpen, K Van Hove, P Gadrat, S Beauceron, S Bernet, C Boudoul, G Bouvier, E Montoya, CAC Chierici, R Contardo, D Courbon, B Depasse, P El Mamouni, H Fan, J Fay, J Gascon, S Gouzevitch, M Ille, B Lagarde, F Laktineh, IB Lethuillier, M Mirabito, L Pequegnot, AL Perries, S Alvarez, JDR Sabes, D Sgandurra, L Sordini, V Donckt, MV Verdier, P Viret, S Toriashvili, T Bagaturia, I Autermann, C Beranek, S Edelhoff, M Feld, L Heister, A Kiesel, MK Klein, K Lipinski, M Ostapchuk, A Preuten, M Raupach, F Schael, S Schulte, JF Verlage, T Weber, H Wittmer, B Zhukov, V Ata, M Brodski, M Dietz-Laursonn, E Duchardt, D Endres, M Erdmann, M Erdweg, S Esch, T Fischer, R Guth, A Hebbeker, T Heidemann, C Hoepfner, K Klingebiel, D Knutzen, S Kreuzer, P Merschmeyer, M Meyer, A Millet, P Olschewski, M Padeken, K Papacz, P Pook, T Radziej, M Reithler, H Rieger, M Scheuch, F Sonnenschein Teyssier, D Thuer, S Cherepanov, V Erdogan, Y Flugge, G Geenen, H Geisler, M Hoehle, F Kargoll, B Kress, T Kuessel, Y Kunsken, A Lingemann, J Nehrkorn, A Nowack, A Nugent, IM Pistone, C Pooth, O Stahl, A Martin, MA Asin, I Bartosik, N Behnke, O Behrens, U Bell, AJ Borras, K Burgmeier, A Cakir, A Campbell, A Choudhury, S Costanza, F Pardos, CD Dolinska, G Dooling, S Dorland, T Eckerlin, G Eckstein, D Eichhorn, T Flucke, G Gallo, E Garcia, JG Geiser, A Gizhko, A Gunnellini, P Hauk, J Hempel, M Jung, H Kalogeropoulos, A Karacheban, O Kasemann, M Katsas, P Kieseler, J Kleinwort, C Korol, I Lange, W Leonard, J Lipka, K Lobanov, A Lohmann, W Mankel, R Marfin, I Melzer-Pellmann, IA Meyer, AB Mittag, G Mnich, J Mussgiller, A Naumann-Emme, S Nayak, A Ntomari, E Perrey, H Pitzl, D Placakyte, R Raspereza, A Roland, B Sahin, MO Saxena, P Schoerner-Sadenius, T Schroder, M Seitz, C Spannagel, S Trippkewitz, KD Walsh, R Wissing, C Blobel, V Vignali, MC Draeger, AR Erfle, J Garutti, E Goebel, K Gonzalez, D Gorner, M Haller, J Hoffmann, M Hoing, RS Junkes, A Klanner, R Kogler, R Lapsien, T Lenz, T 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Papadopoulos, I Paradas, E Strologas, J Bencze, G Hajdu, C Hazi, A Hidas, P Horvath, D Sikler, F Veszpremi, V Vesztergombi, G Zsigmond, AJ Beni, N Czellar, S Karancsi, J Molnar, J Szillasi, Z Bartok, M Makovec, A Raics, P Trocsanyi, ZL Ujvari, B Mal, P Mandal, K Sahoo, DK Sahoo, N Swain, SK Bansal, S Beri, SB Bhatnagar, V Chawla, R Gupta, R Bhawandeep, U Kalsi, AK Kaur, A Kaur, M Kumar, R Mehta, A Mittal, M Singh, JB Walia, G Kumar, A Bhardwaj, A Choudhary, BC Garg, RB Kumar, A Malhotra, S Naimuddin, M Nishu, N Ranjan, K Sharma, R Sharma, V Bhattacharya, S Chatterjee, K Dey, S Dutta, S Jain, S Majumdar, N Modak, A Mondal, K Mukherjee, S Mukhopadhyay, S Roy, A Roy, D Chowdhury, SR Sarkar, S Sharan, M Abdulsalam, A Chudasama, R Dutta, D Jha, V Kumar, V Mohanty, AK Pant, LM Shukla, P Topkar, A Aziz, T Banerjee, S Bhowmik, S Chatterjee, RM Dewanjee, RK Dugad, S Ganguly, S Ghosh, S Guchait, M Gurtu, A Kole, G Kumar, S Mahakud, B Maity, M Majumder, G Mazumdar, K Mitra, S Mohanty, GB Parida, 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Thomas, S. Thomassen, P. Walker, M. Foerster, M. Riley, G. Rose, K. Spanier, S. York, A. Bouhali, O. Hernandez, A. Castaneda Dalchenko, M. De Mattia, M. Delgado, A. Dildick, S. Eusebi, R. Gilmore, J. Kamon, T. Krutelyov, V. Mueller, R. Osipenkov, I. Pakhotin, Y. Patel, R. Perloff, A. Rose, A. Safonov, A. Tatarinov, A. Ulmer, K. A. Akchurin, N. Cowden, C. Damgov, J. Dragoiu, C. Dudero, P. R. Faulkner, J. Kunori, S. Lamichhane, K. Lee, S. W. Libeiro, T. Undleeb, S. Volobouev, I. Appelt, E. Delannoy, A. G. Greene, S. Gurrola, A. Janjam, R. Johns, W. Maguire, C. Mao, Y. Melo, A. Ni, H. Sheldon, P. Snook, B. Tuo, S. Velkovska, J. Xu, Q. Arenton, M. W. Cox, B. Francis, B. Goodell, J. Hirosky, R. Ledovskoy, A. Li, H. Lin, C. Neu, C. Sinthuprasith, T. Sun, X. Wang, Y. Wolfe, E. Wood, J. Xia, F. Clarke, C. Harr, R. Karchin, P. E. Don, C. Kottachchi Kankanamge Lamichhane, P. Sturdy, J. Belknap, D. A. Carlsmith, D. Cepeda, M. Dasu, S. Dodd, L. Duric, S. Friis, E. Gomber, B. Grothe, M. Hall-Wilton, R. Herndon, M. Herve, A. Klabbers, P. Lanaro, A. Levine, A. Long, K. Loveless, R. Mohapatra, A. Ojalvo, I. Perry, T. Pierro, G. A. Polese, G. Ruggles, T. Sarangi, T. Savin, A. Sharma, A. Smith, N. Smith, W. H. Taylor, D. Woods, N. CA CMS Collaboration TI Forward-backward asymmetry of Drell-Yan lepton pairs in pp collisions at root s=8 TeV SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article AB A measurement of the forward-backward asymmetry A(FB) of oppositely charged lepton pairs (mu mu and ee) produced via Z/gamma* boson exchange in pp collisions at root s = 8 TeV is presented. The data sample corresponds to an integrated luminosity of 19.7 fb(-1) collected with the CMS detector at the LHC. The measurement of AFB is performed for dilepton masses between 40 GeV and 2 TeV and for dilepton rapidity up to 5. The AFB measurements as a function of dilepton mass and rapidity are compared with the standard model predictions. 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J.; Vilela Pereira, A.] Univ Estado Rio de Janeiro, Rio De Janeiro, Brazil. [Ahuja, S.; Dogra, S.; Fernandez Perez Tomei, T. R.; Moon, C. S.; Novaes, S. F.; Padula, Sandra S.] Univ Estadual Paulista, Sao Paulo, Brazil. [Bernardes, C. A.; De Souza Santos, A.; Gregores, E. M.; Mercadante, P. G.] Univ Fed ABC, Sao Paulo, Brazil. [Aleksandrov, A.; Hadjiiska, R.; Iaydjiev, P.; Rodozov, M.; Stoykova, S.; Sultanov, G.; Vutova, M.] Inst Nucl Energy Res, Sofia, Bulgaria. [Dimitrov, A.; Glushkov, I.; Litov, L.; Pavlov, B.; Petkov, P.] Univ Sofia, Sofia, Bulgaria. [Ahmad, M.; Bian, J. G.; Chen, G. M.; Chen, H. S.; Chen, M.; Cheng, T.; Du, R.; Jiang, C. H.; Plestina, R.; Romeo, F.; Shaheen, S. M.; Spiezia, A.; Tao, J.; Wang, C.; Wang, Z.; Zhang, H.] Inst High Energy Phys, Beijing, Peoples R China. [Zhang, F.; Asawatangtrakuldee, C.; Ban, Y.; Li, Q.; Liu, S.; Mao, Y.; Qian, S. J.; Wang, D.; Xu, Z.] Peking Univ, State Key Lab Nucl Phys & Technol, Beijing, Peoples R China. [Avila, C.; Cabrera, A.; Chaparro Sierra, L. F.; Florez, C.; Gomez, J. P.; Gomez Moreno, B.; Sanabria, J. C.] Univ Los Andes, Bogota, Colombia. [Godinovic, N.; Lelas, D.; Puljak, I.; Cipriano, P. M. Ribeiro] Univ Split, Fac Elect Engn Mech Engn & Naval Architecture, Split, Croatia. [Antunovic, Z.; Kovac, M.] Univ Split, Fac Sci, Split, Croatia. [Brigljevic, V.; Kadija, K.; Luetic, J.; Micanovic, S.; Sudic, L.] Inst Rudjer Boskov, Zagreb, Croatia. [Attikis, A.; Mavromanolakis, G.; Mousa, J.; Nicolaou, C.; Ptochos, F.; Razis, P. A.; Rykaczewski, H.] Univ Cyprus, Nicosia, Cyprus. [Bodlak, M.; Finger, M.; Finger, M., Jr.] Charles Univ Prague, Prague, Czech Republic. [Assran, Y.; Elgammal, S.; Kamel, A. Ellithi; Mahmoud, M. A.; Mohammed, Y.] Egyptian Network High Energy Phys, Acad Sci Res & Technol Arab Republ Egypt, Cairo, Egypt. [Giammanco, A.; Calpas, B.; Kadastik, M.; Murumaa, M.; Raidal, M.; Tiko, A.; Veelken, C.] NICPB, Tallinn, Estonia. [Eerola, P.; Pekkanen, J.; Voutilainen, M.] Univ Helsinki, Dept Phys, Helsinki, Finland. [Harkonen, J.; Karimaki, V.; Kinnunen, R.; Lampen, T.; Lassila-Perini, K.; Lehti, S.; Linden, T.; Luukka, P.; Maenpaa, T.; Peltola, T.; Tuominen, E.; Tuominiemi, J.; Tuovinen, E.; Wendland, L.] Helsinki Inst Phys, Helsinki, Finland. [Talvitie, J.; Tuuva, T.] Lappeenranta Univ Technol, Lappeenranta, Finland. [Besancon, M.; Couderc, F.; Dejardin, M.; Denegri, D.; Fabbro, B.; Faure, J. L.; Favaro, C.; Ferri, F.; Ganjour, S.; Givernaud, A.; Gras, P.; de Monchenault, G. Hamel; Jarry, P.; Locci, E.; Machet, M.; Malcles, J.; Rander, J.; Rosowsky, A.; Titov, M.; Zghiche, A.] CEA Saclay, DSM IRFU, Gif Sur Yvette, France. [Plestina, R.; Antropov, I.; Baffioni, S.; Beaudette, F.; Busson, P.; Cadamuro, L.; Chapon, E.; Charlot, C.; Dahms, T.; Davignon, O.; Filipovic, N.; Florent, A.; de Cassagnac, R. Granier; Lisniak, S.; Mastrolorenzo, L.; Mine, P.; Naranjo, I. N.; Nguyen, M.; Ochando, C.; Ortona, G.; Paganini, P.; Pigard, P.; Regnard, S.; Salerno, R.; Sauvan, J. B.; Sirois, Y.; Strebler, T.; Yilmaz, Y.; Zabi, A.] Ecole Polytech, IN2P3, Lab Leprince Ringuet, CNRS, Palaiseau, France. [Beluffi, C.; Agram, J. -L.; Andrea, J.; Aubin, A.; Bloch, D.; Brom, J. -M.; Buttignol, M.; Chabert, E. C.; Chanon, N.; Collard, C.; Conte, E.; Coubez, X.; Fontaine, J. -C.; Gele, D.; Goerlach, U.; Goetzmann, C.; Le Bihan, A. -C.; Merlin, J. A.; Skovpen, K.; Van Hove, P.] Univ Haute Alsace Mulhouse, Univ Strasbourg, Inst Pluridisciplinaire Hubert Curien, CNRS IN2P3, Strasbourg, France. [Gadrat, S.] CNRS IN2P3, Ctr Calcul, Inst Natl Phys Nucl & Phys Particules, Villeurbanne, France. [Beauceron, S.; Bernet, C.; Boudoul, G.; Bouvier, E.; Montoya, C. A. Carrillo; Chierici, R.; Contardo, D.; Courbon, B.; Depasse, P.; El Mamouni, H.; Fan, J.; Fay, J.; Gascon, S.; Gouzevitch, M.; Ille, B.; Lagarde, F.; Laktineh, I. B.; Lethuillier, M.; Mirabito, L.; Pequegnot, A. L.; Perries, S.; Alvarez, J. D. Ruiz; Sgandurra, L.; Sordini, V.; Donckt, M. Vander; Verdier, P.; Viret, S.] Univ Lyon 1, Inst Phys Nucl Lyon, CNRS, IN2P3, Villeurbanne, France. [Toriashvili, T.] Georgian Tech Univ, Tbilisi, Rep of Georgia. [Toriashvili, T.; Bagaturia, I.] Tbilisi State Univ, Tbilisi, Rep of Georgia. [Autermann, C.; Beranek, S.; Edelhoff, M.; Feld, L.; Heister, A.; Kiesel, M. K.; Klein, K.; Lipinski, M.; Ostapchuk, A.; Preuten, M.; Raupach, F.; Schael, S.; Schulte, J. F.; Verlage, T.; Weber, H.; Wittmer, B.; Zhukov, V.] Rhein Westfal TH Aachen, Phys Inst 1, Aachen, Germany. [Ata, M.; Brodski, M.; Dietz-Laursonn, E.; Duchardt, D.; Endres, M.; Erdmann, M.; Erdweg, S.; Esch, T.; Fischer, R.; Gueth, A.; Hebbeker, T.; Heidemann, C.; Hoepfner, K.; Klingebiel, D.; Knutzen, S.; Kreuzer, P.; Merschmeyer, M.; Meyer, A.; Millet, P.; Olschewski, M.; Padeken, K.; Papacz, P.; Pook, T.; Radziej, M.; Reithler, H.; Rieger, M.; Scheuch, F.; Sonnenschein; Teyssier, D.; Thueer, S.; Borras, K.; Karacheban, O.] Rhein Westfal TH Aachen, Phys Inst A 3, Aachen, Germany. [Cherepanov, V.; Erdogan, Y.; Fluegge, G.; Geenen, H.; Geisler, M.; Hoehle, F.; Kargoll, B.; Kress, T.; Kuessel, Y.; Kuensken, A.; Lingemann, J.; Nehrkorn, A.; Nowack, A.; Nugent, I. M.; Pistone, C.; Pooth, O.; Stahl, A.] Rhein Westfal TH Aachen, Phys Inst B 3, Aachen, Germany. [Martin, M. Aldaya; Asin, I.; Bartosik, N.; Behnke, O.; Behrens, U.; Bell, A. J.; Borras, K.; Burgmeier, A.; Cakir, A.; Campbell, A.; Choudhury, S.; Costanza, F.; Pardos, C. Diez; Dolinska, G.; Dooling, S.; Dorland, T.; Eckerlin, G.; Eckstein, D.; Eichhorn, T.; Flucke, G.; Gallo, E.; Garcia, J. Garay; Geiser, A.; Gizhko, A.; Gunnellini, P.; Hauk, J.; Hempel, M.; Jung, H.; Kalogeropoulos, A.; Karacheban, O.; Kasemann, M.; Katsas, P.; Kieseler, J.; Kleinwort, C.; Korol, I.; Lange, W.; Leonard, J.; Lipka, K.; Lobanov, A.; Lohmann, W.; Mankel, R.; Marfin, I.; Melzer-Pellmann, I. -A.; Meyer, A. B.; Mittag, G.; Mnich, J.; Mussgiller, A.; Naumann-Emme, S.; Nayak, A.; Ntomari, E.; Perrey, H.; Pitzl, D.; Placakyte, R.; Raspereza, A.; Roland, B.; Sahin, M. Oe.; Saxena, P.; Schoerner-Sadenius, T.; Schroeder, M.; Seitz, C.; Spannagel, S.; Trippkewitz, K. D.; Walsh, R.; Wissing, C.] DESY, Hamburg, Germany. [Gallo, E.; Blobel, V.; Vignali, M. Centis; Draeger, A. R.; Erfle, J.; Garutti, E.; Goebel, K.; Gonzalez, D.; Goerner, M.; Haller, J.; Hoffmann, M.; Hoeing, R. S.; Junkes, A.; Klanner, R.; Kogler, R.; Lapsien, T.; Lenz, T.; Marchesini, I.; Marconi, D.; Meyer, M.; Nowatschin, D.; Ott, J.; Pantaleo, F.; Peiffer, T.; Perieanu, A.; Pietsch, N.; Poehlsen, J.; Rathjens, D.; Sander, C.; Schettler, H.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Schwandt, J.; Sola, V.; Stadie, H.; Steinbrueck, G.; Tholen, H.; Troendle, D.; Usai, E.; Vanelderen, L.; Vanhoefer, A.; Vormwald, B.] Univ Hamburg, Hamburg, Germany. [Akbiyik, M.; Barth, C.; Baus, C.; Berger, J.; Boeser, C.; Butz, E.; Chwalek, T.; Colombo, F.; De Boer, W.; Descroix, A.; Dierlamm, A.; Fink, S.; Frensch, F.; Friese, R.; Giffels, M.; Gilbert, A.; Haitz, D.; Hartmann, F.; Heindl, S. M.; Husemann, U.; Katkov, I.; Kornmayer, A.; Pardo, P. Lobelle; Maier, B.; Mildner, H.; Mozer, M. U.; Mueller, T.; Mueller, Th.; Plagge, M.; Quast, G.; Rabbertz, K.; Roecker, S.; Roscher, F.; Sieber, G.; Simonis, H. J.; Stober, F. M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weber, M.; Weiler, T.; Woehrmann, C.; Wolf, R.] Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Giakoumopoulou, V. A.; Kyriakis, A.; Loukas, D.; Psallidas, A.; Topsis-Giotis, I.] NCSR Demokritos, Inst Nucl & Particle Phys INPP, Aghia Paraskevi, Greece. [Agapitos, A.; Kesisoglou, S.; Panagiotou, A.; Saoulidou, N.; Tziaferi, E.; Sphicas, P.] Univ Athens, Athens, Greece. [Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Loukas, N.; Manthos, N.; Papadopoulos, I.; Paradas, E.; Strologas, J.] Univ Ioannina, Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hazi, A.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.] Wigner Res Ctr Phys, Budapest, Hungary. [Horvath, D.; Beni, N.; Czellar, S.; Karancsi, J.; Molnar, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Karancsi, J.; Bartok, M.; Makovec, A.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, Debrecen, Hungary. [Mal, P.; Mandal, K.; Sahoo, D. K.; Sahoo, N.; Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Bansal, S.; Beri, S. B.; Bhatnagar, V.; Chawla, R.; Gupta, R.; Bhawandeep, U.; Kalsi, A. K.; Kaur, A.; Kaur, M.; Kumar, R.; Mehta, A.; Mittal, M.; Singh, J. B.; Walia, G.] Panjab Univ, Chandigarh, India. [Kumar, Ashok; Bhardwaj, A.; Choudhary, B. C.; Garg, R. B.; Kumar, A.; Malhotra, S.; Naimuddin, M.; Nishu, N.; Ranjan, K.; Sharma, R.; Sharma, V.] Univ Delhi, Delhi, India. [Bhattacharya, S.; Chatterjee, K.; Dey, S.; Dutta, S.; Jain, Sa; Majumdar, N.; Modak, A.; Mondal, K.; Mukherjee, S.; Mukhopadhyay, S.; Roy, A.; Roy, D.; Chowdhury, S. Roy; Sarkar, S.; Sharan, M.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Chudasama, R.; Dutta, D.; Jha, V.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Bombay, Maharashtra, India. [Aziz, T.; Banerjee, S.; Bhowmik, S.; Chatterjee, R. M.; Dewanjee, R. K.; Dugad, S.; Ganguly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Kole, G.; Kumar, S.; Mahakud, B.; Maity, M.; Majumder, G.; Mazumdar, K.; Mitra, S.; Mohanty, G. B.; Parida, B.; Sarkar, T.; Sur, N.; Sutar, B.; Wickramage, N.] Tata Inst Fundamental Res, Bombay, Maharashtra, India. [Chauhan, S.; Dube, S.; Sharma, S.] Indian Inst Sci Educ & Res IISER, Pune, Maharashtra, India. [Bakhshiansohi, H.; Behnamian, H.; Etesami, S. M.; Fahim, A.; Goldouzian, R.; Khakzad, M.; Najafabadi, M. Mohammadi; Naseri, M.; Mehdiabadi, S. Paktinat; Hosseinabadi, F. Rezaei; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Felcini, M.; Grunewald, M.] Univ Coll Dublin, Dublin, Ireland. [Abbrescia, M.; Calabria, C.; Caputo, C.; Colaleo, A.; Creanza, D.; Cristella, L.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; Miniello, G.; My, S.; Nuzzo, S.; Pompili, A.; Pugliese, G.; Radogna, R.; Ranieri, A.; Selvaggi, G.; Silvestris, L.; Venditti, R.; Verwilligen, P.] Univ Coll Dublin, Dublin, Ireland. [Abbrescia, M.; Calabria, C.; Caputo, C.; Cristella, L.; De Palma, M.; Miniello, G.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Silvestris, L.; Venditti, R.; Verwilligen, P.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Chhibra, S. S.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Montanari, A.; Navarria, F. L.; Perrotta, A.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Ist Nazl Fis Nucl, Sez Bologna, Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Chhibra, S. S.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Navarria, F. L.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Cappello, G.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] INFN Sezione Catania, Catania, Italy. [Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.; Viliani, L.] INFN Sez Firenze, Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.; Viliani, L.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Fabbri, F.; Piccolo, D.; Primavera, F.] INFN Lab Nazl Frascati, Frascati, Italy. [Calvelli, V.; Ferro, F.; Lo Vetere, M.; Monge, M. R.; Robutti, E.; Tosi, S.] INFN Sezione Genova, Genoa, Italy. [Calvelli, V.; Lo Vetere, M.; Monge, M. R.; Tosi, S.] Univ Genoa, Genoa, Italy. [Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Malvezzi, S.; Manzoni, R. A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] INFN Sez Milano Bicocca, Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Manzoni, R. A.; Marzocchi, B.; Menasce, D.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Di Guida, S.; Esposito, M.; Fabozzi, F.; Iorio, A. O. M.; Lanza, G.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.; Sciacca, C.] INFN Sez Napoli, Naples, Italy. [Esposito, M.; Iorio, A. O. M.; Sciacca, C.] Univ Napoli Federico II, Naples, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata, Potenza, Italy. [Di Guida, S.; Meola, S.] Univ G Marconi, Rome, Italy. [Azzi, P.; Bacchetta, N.; Benato, L.; Bisello, D.; Boletti, A.; Carlin, R.; Checchia, P.; Dall'Osso, M.; Dorigo, T.; Fantinel, S.; Fanzago, F.; Gasparini, F.; Gasparini, U.; Gonella, F.; Gozzelino, A.; Lacaprara, S.; Margoni, M.; Meneguzzo, A. T.; Montecassiano, F.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] INFN Sez Padova, Padua, Italy. [Benato, L.; Bisello, D.; Boletti, A.; Carlin, R.; Dall'Osso, M.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. Univ Trento, Trento, Italy. [Braghieri, A.; Magnani, A.; Montagna, P.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vai, I.; Vitulo, P.] INFN Sez Pavia, Pavia, Italy. [Montagna, P.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, Pavia, Italy. [Solestizi, L. Alunni; Biasini, M.; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Saha, A.; Santocchia, A.] INFN Sez Perugia, Perugia, Italy. [Solestizi, L. Alunni; Biasini, M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Santocchia, A.] Univ Perugia, Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Foa, L.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] INFN Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Donato, S.; Foa, L.; Ligabue, F.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; D'imperio, G.; Del Re, D.; Diemoz, M.; Gelli, S.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Organtini, G.; Paramatti, R.; Preiato, F.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Traczyk, P.] INFN Sez Roma, Rome, Italy. [Barone, L.; D'imperio, G.; Del Re, D.; Gelli, S.; Longo, E.; Margaroli, F.; Organtini, G.; Preiato, F.; Rahatlou, S.; Santanastasio, F.; Traczyk, P.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Costa, M.; Covarelli, R.; Degano, A.; Demaria, N.; Finco, L.; Kiani, B.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] INFN Sez Torino, Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Costa, M.; Covarelli, R.; Degano, A.; Finco, L.; Kiani, B.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Ruspa, M.] Univ Piemonte Orientale, Novara, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Schizzi, A.; Zanetti, A.] INFN Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Kropivnitskaya, A.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Sakharov, A.; Son, D. C.] Kyungpook Natl Univ, Taegu, South Korea. [Cifuentes, J. A. Brochero; Kim, H.; Kim, T. J.] Chonbuk Natl Univ, Chonju, South Korea. [Song, S.] Chonnam Natl Univ, Inst Univ & Elementary Particles, Kwangju, South Korea. [Choi, S.; Go, Y.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, Y.; Lee, B.; Lee, K.; Lee, K. S.; Lee, S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Yoo, H. D.] Seoul Natl Univ, Seoul, South Korea. [Choi, M.; Kim, H.; Kim, J. H.; Lee, J. S. H.; Park, I. C.; Ryu, G.; Ryu, M. S.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Goh, J.; Kim, D.; Kwon, E.; Lee, J.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.; Vaitkus, J.] Vilnius Univ, Vilnius, Lithuania. [Ahmed, I.; Ibrahim, Z. A.; Komaragiri, J. R.; Ali, M. A. B. Md; Idris, F. Mohamad; Abdullah, W. A. T. Wan; Yusli, M. N.] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Linares, E. Casimiro; Castilla-Valdez, H.; De la Cruz-Burelo, E.; Heredia-De La Cruz, I.; Hernandez-Almada, A.; Lopez-Fernandez, R.; Sanchez-Hernandez, A.] IPN, Ctr Invest & Estudios Avanzados, Mexico City, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Pedraza, I.; Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland, New Zealand. [Butler, P. H.] Univ Canterbury, Christchurch, New Zealand. [Ahmad, A.; Ahmad, M.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Byszuk, A.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.; Walczak, M.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz E Silva, C.; Di Francesco, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Leonardo, N.; Lloret Iglesias, L.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Toldaiev, O.; Vadruccio, D.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Finger, M.; Finger, M., Jr.; Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Shulha, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Kuznetsova, E.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Abdulsalam, A.; Matveev, V.; Andreev, Yu; Dermenev, A.; Gninenko, S.; Golubev, N.; Karneyeu, A.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Musienko, Y.] Inst Nucl Res, Moscow, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Pozdnyakov, I.; Safronov, G.; Spiridonov, A.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow, Russia. [Bylinkin, A.; Azarkin, M.; Dremin, I.; Leonidov, A.] Natl Res Nucl Univ, Moscow Engn Phys Inst MEPhI, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.] PN Lebedev Phys Inst, Moscow, Russia. [Popov, A.; Zhukov, V.; Katkov, I.; Baskakov, A.; Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Myagkov, I.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Lomonosov Moscow State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Snigirev, A.; Adzic, P.; Milosevic, J.; Rekovic, V.] Univ Belgrade, Fac Phys, Belgrade, Serbia. [Adzic, P.; Milosevic, J.; Rekovic, V.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia. [Alcaraz Maestre, J.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.] Ctr Invest Energet Medioambient & Tecnol CIEMAT, Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Palencia Cortezon, E.; Vizan Garcia, J. M.] Univ Oviedo, Oviedo, Spain. [Cabrillo, I. J.; Calderon, A.; Castineiras De Saa, J. R.; De Castro Manzano, P.; Duarte Campderros, J.; Fernandez, M.; Garcia-Ferrero, J.; Gomez, G.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Trevisani, N.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, Santander, Spain. [Rabady, D.; Merlin, J. A.; Lingemann, J.; Pantaleo, F.; Hartmann, F.; Kornmayer, A.; Mohanty, A. K.; Silvestris, L.; Battilana, C.; Viliani, L.; Marzocchi, B.; Di Guida, S.; Meola, S.; Paolucci, P.; Azzi, P.; Dall'Osso, M.; Zucchetta, A.; Ciangottini, D.; Donato, S.; D'imperio, G.; Traczyk, P.; Arcidiacono, R.; Finco, L.; Candelise, V.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Berruti, G. M.; Bloch, P.; Bocci, A.; Bonato, A.; Botta, C.; Breuker, H.; Camporesi, T.; Castello, R.; Cerminara, G.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; Daponte, V.; David, A.; De Gruttola, M.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dorney, B.; du Pree, T.; Duenser, M.; Dupont, N.; Elliott-Peisert, A.; Franzoni, G.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kirschenmann, H.; Kortelainen, M. J.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Lucchini, M. T.; Magini, N.; Malgeri, L.; Mannelli, M.; Martelli, A.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Nemallapudi, M. V.; Neugebauer, H.; Orfanelli, S.; Orsini, L.; Pape, L.; Perez, E.; Peruzzi, M.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Piparo, D.; Racz, A.; Reis, T.; Rolandi, G.; Rovere, M.; Ruan, M.; Sakulin, H.; Schafer, C.; Schwick, C.; Seidel, M.; Sharma, A.; Silva, P.; Simon, M.; Sphicas, P.; Steggemann, J.; Stieger, B.; Stoye, M.; Takahashi, Y.; Treille, D.; Triossi, A.; Tsirou, A.; Veres, G. I.; Wardle, N.; Wohri, H. K.; Zagozdzinska, A.; Zeuner, W. D.; Ulmer, K. A.] CERN, European Org Nucl Res, Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Bani, L.; Bianchini, L.; Casal, B.; Dissertori, G.; Dittmar, M.; Donega, M.; Eller, P.; Grab, C.; Heidegger, C.; Hits, D.; Hoss, J.; Kasieczka, G.; Lustermann, W.; Mangano, B.; Marionneau, M.; del Arbol, P. Martinez Ruiz; Masciovecchio, M.; Meister, D.; Micheli, F.; Musella, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pata, J.; Pauss, F.; Perrozzi, L.; Quittnat, M.; Rossini, M.; Starodumov, A.; Takahashi, M.; Tavolaro, V. R.; Theofilatos, K.; Wallny, R.] ETH, Inst Particle Phys, Zurich, Switzerland. [Aarrestad, T. K.; Amsler, C.; Caminada, L.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Galloni, C.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Ngadiuba, J.; Pinna, D.; Robmann, P.; Ronga, F. J.; Salerno, D.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Doan, T. H.; Jain, Sh; Khurana, R.; Konyushikhin, M.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Yu, S. S.] Natl Cent Univ, Chungli, Taiwan. [Kumar, Arun; Bartek, R.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Fiori, F.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Liu, Y. F.; Lu, R. -S.; Moya, M. Minano; Petrakou, E.; Tsai, J. F.; Tzeng, Y. M.] Natl Taiwan Univ, Taipei, Taiwan. [Asavapibhop, B.; Kovitanggoon, K.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Dept Phys, Fac Sci, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Polatoz, A.; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Akin, I. V.; Bilin, B.; Bilmis, S.; Isildak, B.; Karapinar, G.; Yalvac, M.; Zeyrek, M.] Middle East Tech Univ, Dept Phys, Ankara, Turkey. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Gulmez, E.; Kaya, M.; Kaya, O.; Yetkin, E. A.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cankocak, K.; Sen, S.; Vardarli, F. I.] Istanbul Tech Univ, Istanbul, Turkey. [Grynyov, B.] Natl Acad Sci Ukraine, Inst Scintillat Mat, Kharkov, Ukraine. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Aggleton, R.; Ball, F.; Beck, L.; Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Sakuma, T.; El Nasr-Storey, S. Seif; Senkin, S.; Smith, D.; Smith, V. J.] Univ Bristol, Bristol, Avon, England. [Newbold, D. M.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Calligaris, L.; Cieri, D.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Williams, T.; Womersley, W. J.; Worm, S. D.; Lucas, R.] Rutherford Appleton Lab, Didcot, Oxon, England. [Snigirev, A.; Baber, M.; Bainbridge, R.; Buchmuller, O.; Bundock, A.; Burton, D.; Casasso, S.; Citron, M.; Colling, D.; Corpe, L.; Cripps, N.; Dauncey, P.; Davies, G.; De Wit, A.; Della Negra, M.; Dunne, P.; Elwood, A.; Ferguson, W.; Fulcher, J.; Futyan, D.; Hall, G.; Iles, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Richards, A.; Rose, A.; Seez, C.; Tapper, A.; Uchida, K.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.] Imperial Coll, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge, Middx, England. [Borzou, A.; Call, K.; Dittmann, J.; Hatakeyama, K.; Liu, H.; Pastika, N.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Arcaro, D.; Avetisyan, A.; Bose, T.; Fantasia, C.; Gastler, D.; Lawson, P.; Rankin, D.; Richardson, C.; Rohlf, J.; St John, J.; Sulak, L.; Zou, D.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Berry, E.; Bhattacharya, S.; Cutts, D.; Dhingra, N.; Ferapontov, A.; Garabedian, A.; Hakala, J.; Heintz, U.; Laird, E.; Landsberg, G.; Mao, Z.; Narain, M.; Piperov, S.; Sagir, S.; Syarif, R.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Lander, R.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Cousins, R.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Saltzberg, D.; Takasugi, E.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Paneva, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Negrete, M. Olmedo; Shrinivas, A.; Wei, H.; Wimpenny, S.; Yates, B. R.] Univ Calif Riverside, Riverside, CA 92521 USA. [Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Derdzinski, M.; Holzner, A.; Kelley, R.; Klein, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Tadel, M.; Vartak, A.; Wasserbaech, S.; Welke, C.; Wurthwein, F.; Yagil, A.; Della Porta, G. Zevi] Univ Calif San Diego, La Jolla, CA 92093 USA. [Bradmiller-Feld, J.; Campagnari, C.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Gran, J.; Incandela, J.; Mccoll, N.; Mullin, S. D.; Richman, J.; Stuart, D.; Suarez, I.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dubinin, M.; Anderson, D.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Pierini, M.; Spiropulu, M.; Vlimant, J. R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Andrews, M. B.; Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Paulini, M.; Russ, J.; Sun, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Jensen, F.; Johnson, A.; Krohn, M.; Mulholland, T.; Nauenberg, U.; Stenson, K.; Wagner, S. R.] Univ Colorado Boulder, Boulder, CO USA. [Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Rinkevicius, A.; Ryd, A.; Skinnari, L.; Soffi, L.; Sun, W.; Tan, S. M.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Banerjee, S.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Grunendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hasegawa, S.; Hirschauer, J.; Hu, Z.; Jindariani, S.; Johnson, M.; Joshi, U.; Jung, A. W.; Klima, B.; Kreis, B.; Kwan, S.; Lammel, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; De Sa, R. Lopes; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mishra, K.; Mrenna, S.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Pedro, K.; Prokofyev, O.; Rakness, G.; Sexton-Kennedy, E.; Soha, A.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vernieri, C.; Verzocchi, M.; Vidal, R.; Weber, H. A.; Whitbeck, A.; Yang, F.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Carnes, A.; Carver, M.; Curry, D.; Das, S.; Di Giovanni, G. P.; Field, R. D.; Furic, I. K.; Gleyzer, S. V.; Hugon, J.; Konigsberg, J.; Korytov, A.; Low, J. F.; Ma, P.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Rank, D.; Rossin, R.; Shchutska, L.; Snowball, M.; Sperka, D.; Terentyev, N.; Thomas, L.; Wang, J.; Wang, S.; Yelton, J.] Univ Florida, Gainesville, FL USA. [Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Ackert, A.; Adams, J. R.; Adams, T.; Askew, A.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Khatiwada, A.; Prosper, H.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Bhopatkar, V.; Colafranceschi, S.; Hohlmann, M.; Kalakhety, H.; Noonan, D.; Roy, T.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Kurt, P.; O'Brien, C.; Gonzalez, I. D. Sandoval; Silkworth, C.; Turner, P.; Varelas, N.; Wu, Z.; Zakaria, M.] Univ Illinois Chicago UIC, Chicago, IL USA. [Bilki, B.; Clarida, W.; Dilsiz, K.; Durgut, S.; Gandrajula, R. P.; Haytmyradov, M.; Khristenko, V.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Snyder, C.; Tiras, E.; Wetzel, J.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Anderson, I.; Barnett, B. A.; Blumenfeld, B.; Cocoros, A.; Eminizer, N.; Fehling, D.; Feng, L.; Gritsan, A. V.; Maksimovic, P.; Osherson, M.; Roskes, J.; Sarica, U.; Swartz, M.; Xiao, M.; Xin, Y.; You, C.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Bruner, C.; Kenny, R. P., III; Majumder, D.; Malek, M.; Murray, M.; Sanders, S.; Stringer, R.; Wang, Q.] Univ Kansas, Lawrence, KS 66045 USA. [Ivanov, A.; Kaadze, K.; Khalil, S.; Makouski, M.; Maravin, Y.; Mohammadi, A.; Saini, L. K.; Skhirtladze, N.; Toda, S.] Kansas State Univ, Manhattan, KS 66506 USA. [Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Anelli, C.; Baden, A.; Baron, O.; Belloni, A.; Calvert, B.; Eno, S. C.; Ferraioli, C.; Gomez, J. A.; Hadley, N. J.; Jabeen, S.; Kellogg, R. G.; Kolberg, T.; Kunkle, J.; Lu, Y.; Mignerey, A. C.; Shin, Y. H.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Baty, A.; Bierwagen, K.; Brandt, S.; Busza, W.; Cali, I. A.; Demiragli, Z.; Di Matteo, L.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Iiyama, Y.; Innocenti, G. M.; Klute, M.; Kovalskyi, D.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Marini, A. C.; Mcginn, C.; Mironov, C.; Narayanan, S.; Niu, X.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Salfeld-Nebgen, J.; Stephans, G. S. F.; Sumorok, K.; Varma, M.; Velicanu, D.; Veverka, J.; Wang, J.; Wang, T. W.; Wyslouch, B.; Yang, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Snigirev, A.; Dahmes, B.; Evans, A.; Finkel, A.; Gude, A.; Hansen, P.; Kalafut, S.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Lesko, Z.; Mans, J.; Nourbakhsh, S.; Ruckstuhl, N.; Rusack, R.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Fangmeier, C.; Suarez, R. Gonzalez; Kamalieddin, R.; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Meier, F.; Monroy, J.; Ratnikov, F.; Siado, J. E.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Alyari, M.; Dolen, J.; George, J.; Godshalk, A.; Harrington, C.; Iashvili, I.; Kaisen, J.; Kharchilava, A.; Kumar, A.; Rappoccio, S.; Roozbahani, B.] SUNY Buffalo, Buffalo, NY 14620 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Hortiangtham, A.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; De Lima, R. Teixeira; Trocino, D.; Wang, R. -J.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Hahn, K. A.; Kubik, A.; Low, J. F.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Trovato, M.; Velasco, M.] Northwestern Univ, Evanston, IL USA. [Snigirev, A.; Brinkerhoff, A.; Dev, N.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Lynch, S.; Marinelli, N.; Meng, F.; Mueller, C.; Musienko, Y.; Pearson, T.; Planer, M.; Reinsvold, A.; Ruchti, R.; Smith, G.; Taroni, S.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hart, A.; Hill, C.; Hughes, R.; Ji, W.; Kotov, K.; Ling, T. Y.; Liu, B.; Luo, W.; Puigh, D.; Rodenburg, M.; Winer, B. L.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Driga, O.; Elmer, P.; Hardenbrook, J.; Hebda, P.; Koay, S. 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RI Azarkin, Maxim/N-2578-2015; Kirakosyan, Martin/N-2701-2015; Della Ricca, Giuseppe/B-6826-2013; Puljak, Ivica/D-8917-2017; TUVE', Cristina/P-3933-2015; Goh, Junghwan/Q-3720-2016; Varela, Joao/K-4829-2016; Lokhtin, Igor/D-7004-2012; Paulini, Manfred/N-7794-2014; Smirnov, Vitaly/B-5001-2017; Moraes, Arthur/F-6478-2010; Ogul, Hasan/S-7951-2016; Dremin, Igor/K-8053-2015; Govoni, Pietro/K-9619-2016; Manganote, Edmilson/K-8251-2013; Andreev, Vladimir/M-8665-2015; Konecki, Marcin/G-4164-2015; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Leonidov, Andrey/M-4440-2013 OI Della Ricca, Giuseppe/0000-0003-2831-6982; TUVE', Cristina/0000-0003-0739-3153; Goh, Junghwan/0000-0002-1129-2083; Varela, Joao/0000-0003-2613-3146; Paulini, Manfred/0000-0002-6714-5787; Moraes, Arthur/0000-0002-5157-5686; Ogul, Hasan/0000-0002-5121-2893; Govoni, Pietro/0000-0002-0227-1301; Konecki, Marcin/0000-0001-9482-4841; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; FU Marie-Curie program; European Research Council; EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS program of the Foundation for Polish Science; European Union, Regional Development Fund; OPUS program of the National Science Center (Poland); Compagnia di San Paolo (Torino); MIUR (Italy) [20108T4XTM]; Thalis program - EU-ESF; Aristeia program - EU-ESF; Greek NSRF; National Priorities Research Program by Qatar National Research Fund; Rachadapisek Sompot Fund for Postdoctoral Fellowship; Chulalongkorn University (Thailand); Chulalongkorn Academic into Its second Century Project Advancement Project (Thailand); Welch Foundation [C-1845] FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWFW and FWF (Austria); FNRS and FWO(Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES and CSF (Croatia); RPF (Cyprus); MoER, ERCIUT and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NIH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); MSIP and NRF (Republic of Korea); LAS (Lithuania); MOE and UM (Malaysia); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Dubna); MON, RosAtom, RAS and RFBR (Russia); MESTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter, IPST, STAR and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU and SFFR (Ukraine); STFC (United Kingdom); DOE and NSF (USA). Individuals have received support from the Marie-Curie program and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS program of the Foundation for Polish Science, cofinanced from European Union, Regional Development Fund; the OPUS program of the National Science Center (Poland); the Compagnia di San Paolo (Torino); MIUR project 20108T4XTM (Italy); the Thalis and Aristeia programs cofinanced by EU-ESF and the Greek NSRF; the National Priorities Research Program by Qatar National Research Fund; the Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); the Chulalongkorn Academic into Its second Century Project Advancement Project (Thailand); and the Welch Foundation, contract C-1845. NR 45 TC 3 Z9 3 U1 24 U2 24 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD JUN 14 PY 2016 VL 76 IS 6 AR 325 DI 10.1140/epjc/s10052-016-4156-z PG 24 WC Physics, Particles & Fields SC Physics GA DZ7HZ UT WOS:000386036800001 PM 28280439 ER PT J AU Aaboud, M Aad, G Abbott, B Abdallah, J Abdinov, O Abeloos, B Aben, R AbouZeid, OS Abraham, NL Abramowicz, H Abreu, H Abreu, R Abulaitia, Y Aba, BSA Adamczyka, L Adams, DL Adelman, J Adomeitioi, S Adye, T Affolder, AA Agatonovic-Jovin, T Agricola, J Aguilar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TPA Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Aliev, M Alimonti, G Alison, J Alkire, SP Allbrooke, BMM Allen, BW Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Alstaty, M Gonzalez, BA Piqueras, DA Alviggi, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorirn, A Amoroso, S Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anders, JK Anderson, KJ 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